WorldWideScience

Sample records for antiferromagnetic spin correlations

  1. Antiferromagnetic phase transition and spin correlations in NiO

    DEFF Research Database (Denmark)

    Chatterji, Tapan; McIntyre, G.J.; Lindgård, Per-Anker

    2009-01-01

    We have investigated the antiferromagnetic (AF) phase transition and spin correlations in NiO by high-temperature neutron diffraction below and above TN. We show that AF phase transition is a continuous second-order transition within our experimental resolution. The spin correlations manifested...... by this process. We determined the critical exponents =0.328±0.002 and =0.64±0.03 and the Néel temperature TN=530±1 K. These critical exponents suggest that NiO should be regarded as a 3dXY system...

  2. Excitations and spin correlations near the interface of two three-dimensional Heisenberg antiferromagnets

    Energy Technology Data Exchange (ETDEWEB)

    Voropajeva, N., E-mail: niina.voropajeva@ut.ee [Institute of Physics, University of Tartu, Riia 142, 51014 Tartu (Estonia); Sherman, A., E-mail: alexei@fi.tartu.ee [Institute of Physics, University of Tartu, Riia 142, 51014 Tartu (Estonia)

    2012-09-03

    Magnetic excitations and spin correlations near the interface of two spin-1/2 Heisenberg antiferromagnets are considered using the spin-wave approximation. When the interaction between boundary spins differs essentially from exchange constants inside the antiferromagnets, quasi-two-dimensional spin waves appear in the near-boundary region. They eject bulk magnons from this region, thereby dividing the antiferromagnets into areas with different magnetic excitations. The decreased dimensionality of the near-boundary modes leads to amplified nearest-neighbor spin correlations in the interface area. -- Highlights: ► Excitations near the interface of two Heisenberg antiferromagnets are considered. ► Different quasi-two-dimensional spin waves may appear in the interface region. ► The interface modes eject bulk modes from the near-boundary region. ► The interface modes produce amplified spin correlations near the boundary.

  3. Magnetic correlations and quantum criticality in the insulating antiferromagnetic, insulating spin liquid, renormalized Fermi liquid, and metallic antiferromagnetic phases of the Mott system V2O3

    Science.gov (United States)

    Bao, Wei; Broholm, C.; Aeppli, G.; Carter, S. A.; Dai, P.; Rosenbaum, T. F.; Honig, J. M.; Metcalf, P.; Trevino, S. F.

    1998-11-01

    Magnetic correlations in all four phases of pure and doped vanadium sesquioxide (V2O3) have been examined by magnetic thermal-neutron scattering. Specifically, we have studied the antiferromagnetic and paramagnetic phases of metallic V2-yO3, the antiferromagnetic insulating and paramagnetic metallic phases of stoichiometric V2O3, and the antiferromagnetic and paramagnetic phases of insulating V1.944Cr0.056O3. While the antiferromagnetic insulator can be accounted for by a localized Heisenberg spin model, the long-range order in the antiferromagnetic metal is an incommensurate spin-density wave, resulting from a Fermi surface nesting instability. Spin dynamics in the strongly correlated metal are dominated by spin fluctuations with a ``single lobe'' spectrum in the Stoner electron-hole continuum. Furthermore, our results in metallic V2O3 represent an unprecedentedly complete characterization of the spin fluctuations near a metallic quantum critical point, and provide quantitative support for the self-consistent renormalization theory for itinerant antiferromagnets in the small moment limit. Dynamic magnetic correlations for ħωantiferromagnetic insulator, from the paramagnetic metal and the paramagnetic insulator, introduces a sudden switching of magnetic correlations to a different spatial periodicity which indicates a sudden change in the underlying spin Hamiltonian. To describe this phase transition and also the unusual short-range order in the paramagnetic state, it seems necessary to take into account the orbital degrees of freedom associated with the degenerate d orbitals at the Fermi level in V2O3.

  4. Antiferromagnetic spin-orbitronics

    KAUST Repository

    Manchon, Aurelien

    2015-05-01

    Antiferromagnets have long remained an intriguing and exotic state of matter, whose application has been restricted to enabling interfacial exchange bias in metallic and tunneling spin-valves [1]. Their role in the expanding field of applied spintronics has been mostly passive and the in-depth investigation of their basic properties mostly considered from a fundamental perspective.

  5. Antiferromagnetic spin Seebeck effect.

    Energy Technology Data Exchange (ETDEWEB)

    Wu, Stephen M.; Zhang, Wei; KC, Amit; Borisov, Pavel; Pearson, John E.; Jiang, J. Samuel; Lederman, David; Hoffmann, Axel; Bhattacharya, Anand

    2016-03-03

    We report on the observation of the spin Seebeck effect in antiferromagnetic MnF2. A device scale on-chip heater is deposited on a bilayer of MnF2 (110) (30nm)/Pt (4 nm) grown by molecular beam epitaxy on a MgF2(110) substrate. Using Pt as a spin detector layer, it is possible to measure the thermally generated spin current from MnF2 through the inverse spin Hall effect. The low temperature (2–80 K) and high magnetic field (up to 140 kOe) regime is explored. A clear spin-flop transition corresponding to the sudden rotation of antiferromagnetic spins out of the easy axis is observed in the spin Seebeck signal when large magnetic fields (>9T) are applied parallel to the easy axis of the MnF2 thin film. When the magnetic field is applied perpendicular to the easy axis, the spin-flop transition is absent, as expected.

  6. Antiferromagnetic Spin Seebeck Effect

    Science.gov (United States)

    Wu, Stephen M.; Zhang, Wei; KC, Amit; Borisov, Pavel; Pearson, John E.; Jiang, J. Samuel; Lederman, David; Hoffmann, Axel; Bhattacharya, Anand

    2016-03-01

    We report on the observation of the spin Seebeck effect in antiferromagnetic MnF2 . A device scale on-chip heater is deposited on a bilayer of MnF2 (110) (30 nm )/Pt (4 nm) grown by molecular beam epitaxy on a MgF2 (110) substrate. Using Pt as a spin detector layer, it is possible to measure the thermally generated spin current from MnF2 through the inverse spin Hall effect. The low temperature (2-80 K) and high magnetic field (up to 140 kOe) regime is explored. A clear spin-flop transition corresponding to the sudden rotation of antiferromagnetic spins out of the easy axis is observed in the spin Seebeck signal when large magnetic fields (>9 T ) are applied parallel to the easy axis of the MnF2 thin film. When the magnetic field is applied perpendicular to the easy axis, the spin-flop transition is absent, as expected.

  7. Antiferromagnetic spin Seebeck Effect

    OpenAIRE

    Wu, SM; W. Zhang; Kc, A; Borisov, P.; Pearson, JE; Jiang, JS; Lederman, D.; Hoffmann, A.; Bhattacharya, A

    2015-01-01

    We report on the observation of the spin Seebeck effect in antiferromagnetic MnF_{2}. A device scale on-chip heater is deposited on a bilayer of MnF_{2} (110) (30  nm)/Pt (4 nm) grown by molecular beam epitaxy on a MgF_{2} (110) substrate. Using Pt as a spin detector layer, it is possible to measure the thermally generated spin current from MnF_{2} through the inverse spin Hall effect. The low temperature (2-80 K) and high magnetic field (up to 140 kOe) regime is explored. A clear spin-flop t...

  8. Spin dynamics and magnetic correlation length in two-dimensional quantum heisenberg antiferromagnets

    Science.gov (United States)

    Carretta; Ciabattoni; Cuccoli; Mognaschi; Rigamonti; Tognetti; Verrucchi

    2000-01-10

    The correlated spin dynamics and temperature dependence of the correlation length xi(T) in two-dimensional quantum (S = 1/2) Heisenberg antiferromagnets (2DQHAF) on a square lattice are discussed in light of experimental results of proton spin lattice relaxation in copper formiate tetradeuterate. In this compound the exchange constant is much smaller than the one in recently studied 2DQHAF, such as La2CuO4 and Sr2CuO2Cl2. Thus the spin dynamics can be probed in detail over a wider temperature range. The NMR relaxation rates turn out to be in excellent agreement with a theoretical mode-coupling calculation. The deduced temperature behavior of xi(T) is in agreement with high-temperature expansions, quantum Monte Carlo simulations, and the pure quantum self-consistent harmonic approximation. Contrary to the predictions of the theories based on the nonlinear sigma model, no evidence of crossover between different quantum regimes is observed.

  9. A spin-1 kagome antiferromagnet

    Science.gov (United States)

    Tovar, Mayra; Shtengel, Kirill; Refael, Gil

    2010-03-01

    We study a spin-1 antiferromagnet on the kagom'e lattice. We start by constructing a Klein-type SU(2) symmetric Hamiltonian which contains Heisenberg interactions between nearest and next-nearest neighbors as well as three-body terms. Our model Hamiltonian has an extensive degenerate ground state whose manifold is spanned by the AKLT-like valence bond states. We also perturb the parent Hamiltonian by introducing an enhancement to the nearest neighbor antiferromagnetic Heisenberg interactions. By projecting this perturbation onto the basis spanned by the unperturbed ground states, we derive an effective Hamiltonian which is dual to that of the transverse field antiferromagnetic Ising model on the triangular lattice. Based on the parameters of our model, we find it to be in the order-by-disorder phase. The ground state is a valence bond crystal stabilized by quantum fluctuations. We also discuss excitations, both magnetic and non-magnetic, and address their possible relevance to experiment.

  10. Antiferromagnetic noise correlations in optical lattices

    DEFF Research Database (Denmark)

    Bruun, Niels Bohr International Academy, University of Copenhagen, DK-2100 Copenhagen Ø, Denmark, Georg Morten; Syljuåsen, F. T.; Pedersen, K. G. L.;

    2009-01-01

    We analyze how noise correlations probed by time-of-flight experiments reveal antiferromagnetic (AF) correlations of fermionic atoms in two-dimensional and three-dimensional optical lattices. Combining analytical and quantum Monte Carlo calculations using experimentally realistic parameters, we...... show that AF correlations can be detected for temperatures above and below the critical temperature for AF ordering. It is demonstrated that spin-resolved noise correlations yield important information about the spin ordering. Finally, we show how to extract the spin correlation length and the related...

  11. Superconductivity, Antiferromagnetism, and Kinetic Correlation in Strongly Correlated Electron Systems

    Directory of Open Access Journals (Sweden)

    Takashi Yanagisawa

    2015-01-01

    Full Text Available We investigate the ground state of two-dimensional Hubbard model on the basis of the variational Monte Carlo method. We use wave functions that include kinetic correlation and doublon-holon correlation beyond the Gutzwiller ansatz. It is still not clear whether the Hubbard model accounts for high-temperature superconductivity. The antiferromagnetic correlation plays a key role in the study of pairing mechanism because the superconductive phase exists usually close to the antiferromagnetic phase. We investigate the stability of the antiferromagnetic state when holes are doped as a function of the Coulomb repulsion U. We show that the antiferromagnetic correlation is suppressed as U is increased exceeding the bandwidth. High-temperature superconductivity is possible in this region with enhanced antiferromagnetic spin fluctuation and pairing interaction.

  12. Antiferromagnetic spin ordering and interlayer magnetic correlations in MnTe/CdTe superlattices

    Science.gov (United States)

    Giebultowicz, T. M.; Faschinger, W.; Nunez, V.; Klosowski, P.; Bauer, G.; Sitter, H.; Furdyna, J. K.

    1994-04-01

    Results of neutron scattering studies on MnTe/CdTe superlattices with ultrathin non-magnetic CdTe "barriers" are presented and compared with data from earlier studies on MnSe/ZnSe, MnTe/ZnTe, and MnSe/ZnTe multilayers with thick non-magnetic spacers. The experiments revealed two qualitatively new effects—namely, (i) the existence of pronounced interlayer magnetic correlations in the case of the CdTe thickness corresponding to two single monolayers and (ii) the coexistence of two magnetic phases that never occurred simultaneously in the previously studied systems.

  13. Paramagnetic and Antiferromagnetic Spin Seebeck Effect

    Science.gov (United States)

    Wu, Stephen

    We report on the observation of the longitudinal spin Seebeck effect in both antiferromagnetic and paramagnetic insulators. By using a microscale on-chip local heater, it is possible to generate a large thermal gradient confined to the chip surface without a large increase in the total sample temperature. This technique allows us to easily access low temperatures (200 mK) and high magnetic fields (14 T) through conventional dilution refrigeration and superconducting magnet setups. By exploring this regime, we detect the spin Seebeck effect through the spin-flop transition in antiferromagnetic MnF2 when a large magnetic field (>9 T) is applied along the easy axis direction. Using the same technique, we are also able to resolve a spin Seebeck effect from the paramagnetic phase of geometrically frustrated antiferromagnet Gd3Ga5O12 (gadolinium gallium garnet) and antiferromagnetic DyScO3 (DSO). Since these measurements occur above the ordering temperatures of these two materials, short-range magnetic order is implicated as the cause of the spin Seebeck effect in these systems. The discovery of the spin Seebeck effect in these two materials classes suggest that both antiferromagnetic spin waves and spin excitations from short range magnetic order may be used to generate spin current from insulators and that the spin wave spectra of individual materials are highly important to the specifics of the longitudinal spin Seebeck effect. Since insulating antiferromagnets and paramagnets are far more common than the typical insulating ferrimagnetic materials used in spin Seebeck experiments, this discovery opens up a large new class of materials for use in spin caloritronic devices. All authors acknowledge support of the U.S. Department of Energy (DOE), Office of Science, Basic Energy Sciences (BES), Materials Sciences and Engineering Division. The use of facilities at the Center for Nanoscale Materials, was supported by the U.S. DOE, BES under Contract No. DE-AC02-06CH11357.

  14. Antiferromagnetic domain wall motion driven by spin-orbit torques

    Science.gov (United States)

    Shiino, Takayuki; Oh, Se-Hyeok; Haney, Paul M.; Lee, Seo-Won; Go, Gyungchoon; Park, Byong-Guk; Lee, Kyung-Jin

    2016-01-01

    We theoretically investigate dynamics of antiferromagnetic domain walls driven by spin-orbit torques in antiferromagnet/heavy metal bilayers. We show that spin-orbit torques drive antiferromagnetic domain walls much faster than ferromagnetic domain walls. As the domain wall velocity approaches the maximum spin-wave group velocity, the domain wall undergoes Lorentz contraction and emits spin-waves in the terahertz frequency range. The interplay between spin-orbit torques and the relativistic dynamics of antiferromagnetic domain walls leads to the efficient manipulation of antiferromagnetic spin textures and paves the way for the generation of high frequency signals from antiferromagnets. PMID:27588878

  15. Spin transfer in antiferromagnets (Conference Presentation)

    Science.gov (United States)

    Moriyama, Takahiro

    2016-10-01

    Since antiferromagnets (AFMs) have no spontaneous magnetization unlike ferromagnetic materials, it is not easy to manipulate the magnetic moments in AFMs by external magnetic field. However, recent theoretical studies suggest that it is possible to manipulate the magnetization in AFMs by spin-transfer-torque in a similar manner to ferromagnetic materials. In this study, we perform spin-toque ferromagnetic resonance (ST-FMR) measurements on FeNi/NiO/Pt multilayers to experimentally investigate the interaction between the spin current and the magnetic moments of antiferromagnetic NiO. The spin current is injected to the NiO by the spin Hall effect in Pt. The monotonous change in the FMR linewidth of this system with respect to the spin current can be interpreted in a way that the spin current is transferred through the NiO and interacts with the FeNi. This intriguing spin current transport can be explained by the angular momentum transfer mediated by the antiferromagnetic magnons. The results assure that the spin current exerts a torque on the NiO magnetic moments and excites their dynamics. In the talk, recent results will be also discussed.

  16. Spin-Mechanical Inertia in Antiferromagnet

    OpenAIRE

    2016-01-01

    The conservation of angular momentum has served as a guiding principle in the coupled dynamics of quantum spins and mechanical rotations. However, in an antiferromagnet with vanishing magnetization, new fundamental rules are required to properly describe spin-mechanical phenomena. Here we demonstrate that the Neel order dynamics affects the mechanical motion of a rigid body by modifying its inertia tensor in the presence of strong magnetocrystalline anisotropy. This effect depends on temperat...

  17. Spin-transfer torque induced spin waves in antiferromagnetic insulators

    Science.gov (United States)

    Daniels, Matthew; Guo, Wei; Stocks, G. Malcolm; Xiao, Di; Xiao, Jiang

    2015-03-01

    We explore the possibility of exciting spin waves in insulating antiferromagnetic films by injecting spin current at the surface. We analyze both magnetically compensated and uncompensated interfaces. We find that the spin current induced spin-transfer torque can excite spin waves in insulating antiferromagnetic materials and that the chirality of the excited spin wave is determined by the polarization of the injected spin current. Furthermore, the presence of magnetic surface anisotropy can greatly increase the accessibility of these excitations. Supported by NSF EFRI-1433496 (M.W.D), U.S. DOE Office of Basic Energy Sciences, Materials Sciences and Engineering (D.X. & G.M.S.), Major State Basic Research Project of China and National Natural Science Foundation of China (W.G. and J.X.).

  18. Spin Transport in Ferromagnetic and Antiferromagnetic Textures

    KAUST Repository

    Akosa, Collins A.

    2016-12-07

    In this dissertation, we provide an accurate description of spin transport in magnetic textures and in particular, we investigate in detail, the nature of spin torque and magnetic damping in such systems. Indeed, as will be further discussed in this thesis, the current-driven velocity of magnetic textures is related to the ratio between the so-called non-adiabatic torque and magnetic damping. Uncovering the physics underlying these phenomena can lead to the optimal design of magnetic systems with improved efficiency. We identified three interesting classes of systems which have attracted enormous research interest (i) Magnetic textures in systems with broken inversion symmetry: We investigate the nature of magnetic damping in non-centrosymmetric ferromagnets. Based on phenomenological and microscopic derivations, we show that the magnetic damping becomes chiral, i.e. depends on the chirality of the magnetic texture. (ii) Ferromagnetic domain walls, skyrmions and vortices: We address the physics of spin transport in sharp disordered magnetic domain walls and vortex cores. We demonstrate that upon spin-independent scattering, the non-adiabatic torque can be significantly enhanced. Such an enhancement is large for vortex cores compared to transverse domain walls. We also show that the topological spin currents owing in these structures dramatically enhances the non-adiabaticity, an effect unique to non-trivial topological textures (iii) Antiferromagnetic skyrmions: We extend this study to antiferromagnetic skyrmions and show that such an enhanced topological torque also exist in these systems. Even more interestingly, while such a non-adiabatic torque inuences the undesirable transverse velocity of ferromagnetic skyrmions, in antiferromagnetic skyrmions, the topological non-adiabatic torque directly determines the longitudinal velocity. As a consequence, scaling down the antiferromagnetic skyrmion results in a much more efficient spin torque.

  19. High-Tc spin superfluidity in antiferromagnets.

    Science.gov (United States)

    Bunkov, Yu M; Alakshin, E M; Gazizulin, R R; Klochkov, A V; Kuzmin, V V; L'vov, V S; Tagirov, M S

    2012-04-27

    We report the observation of the unusual behavior of induction decay signals in antiferromagnetic monocrystals with Suhl-Nakamura interactions. The signals show the formation of the Bose-Einstein condensation (BEC) of magnons and the existence of spin supercurrent, in complete analogy with the spin superfluidity in the superfluid (3)He and the atomic BEC of quantum gases. In the experiments described here, the temperature of the magnon BEC is a thousand times larger than in the superfluid (3)He. It opens a possibility to apply the spin supercurrent for various magnetic spintronics applications.

  20. Transformation of spin current by antiferromagnetic insulators

    Science.gov (United States)

    Khymyn, Roman; Lisenkov, Ivan; Tiberkevich, Vasil S.; Slavin, Andrei N.; Ivanov, Boris A.

    2016-06-01

    It is demonstrated theoretically that a thin layer of an anisotropic antiferromagnetic (AFM) insulator can effectively conduct spin current through the excitation of a pair of evanescent AFM spin wave modes. The spin current flowing through the AFM is not conserved due to the interaction between the excited AFM modes and the AFM lattice and, depending on the excitation conditions, can be either attenuated or enhanced. When the phase difference between the excited evanescent modes is close to π /2 , there is an optimum AFM thickness for which the output spin current reaches a maximum, which can significantly exceed the magnitude of the input spin current. The spin current transfer through the AFM depends on the ambient temperature and increases substantially when temperature approaches the Néel temperature of the AFM layer.

  1. Spin structures in antiferromagnetic nanoparticles

    DEFF Research Database (Denmark)

    Brok, Erik

    in aqueous suspension was controlled by a hydrothermal treatment and by changing the ionic strenght of the suspension. Interestingly addition of NaCl to the suspension resulted in the particles aggregating in long linear chains, with neighbouring particles aligned along a common [001] axis of the hexagonal......, proposed to explain the unusual magnetic properties of the mineral. In summary the thesis have demonstrated methods for investigation of spin structures in magnetic nanoparticles. In particular, the classical model of the temperature dependence of canted spin structures sucessfully explains many...

  2. Spin Seebeck Effect Signals from Antiferromagnets

    Science.gov (United States)

    Prakash, Arati; Brangham, Jack; Yang, Fengyuan; Heremans, Joseph

    The Longitudinal Spin Seebeck Effect (LSSE), in which a heat current stimulates spin propagation across an interface between a magnetic material and a normal metal, is well established and observed in ferromagnetic systems. Data have been presented indicating that antiferromagnetic systems could also give rise to LSSE signals. We report here on LSSE signal measured on the Pt/NiO/YIG structure, where NiO is an antiferromagnet. This system is reported to exhibit antiferromagnonic transport. We explore the dependence of the signal on the thickness of the NiO and YIG layers. We also report its temperature dependence, which was not explored before. The results are interpreted in terms of the temperature dependence of the magnon density of states. It appears that magnon modes with energies below about 40 K are most involved in the process, as was the case to the LSSE on YIG itself. Preliminary results using other antiferromagnets and other inverse spin-Hall layers look promising and will also be reported Work supported by ARO- MURI W911NF-14-1-0016.

  3. Antiferromagnetic spin wave and the superconductivity

    Science.gov (United States)

    Koh, Shun-ichiro

    2000-07-01

    The neutron scattering of UPd 2Al 3 showed that a sharp peak, which is absent in the normal phase, appears in the superconducting phase (Metoki et al., J. Phys. Soc. Japan 66 (1997) 2560; Bernhoeft et al., Phys. Rev. Lett. 81 (1998) 4244). Assuming this excitation to be an antiferromagnetic (AFM) spin-wave, this paper deals with its enhancement by the superconductivity. Applying the slave-boson formalism, we consider the AFM ordering as a spin-density-wave (Koh, Phys. Lett. A 253 (1999) 98). Above Tc, the spin-wave suffers an energy dissipation due to the conduction electron. Below Tc, the superconductivity suppresses the dissipation, resulting in the growth of the AFM spin-wave.

  4. High-field spin dynamics of antiferromagnetic quantum spin chains

    DEFF Research Database (Denmark)

    Enderle, M.; Regnault, L.P.; Broholm, C.;

    2000-01-01

    The characteristic internal order of macroscopic quantum ground states in one-dimensional spin systems is usually not directly accessible, but reflected in the spin dynamics and the field dependence of the magnetic excitations. In high magnetic fields quantum phase transitions are expected. We...... present recent work on the high-field spin dynamics of the S = I antiferromagnetic Heisenberg chains NENP (Haldane ground state) and CsNiCl3 (quasi-1D HAF close to the quantum critical point), the uniform S = 1/2 chain CTS, and the spin-Peierls system CuGeO3. (C) 2000 Elsevier Science B,V. All rights...

  5. Spin dynamics in geometrically frustrated antiferromagnetic pyrochlores

    Science.gov (United States)

    Gardner, J. S.; Ehlers, G.; Bramwell, S. T.; Gaulin, B. D.

    2004-03-01

    We have studied the spin dynamics of several antiferromagnetic pyrochlore oxides. These magnets are geometrically frustrated and only reach their ground states at temperatures much lower than that expected from mean field theory. Here we present data on the magnetic nature, especially the spin dynamics of Tb2Ti2O7, Gd2Ti2O7 and Y2Mo2O7. In these systems the ground states are found to be very different. Y2Mo2O7 freezes completely into a spin glass-like state, Tb2Ti2O7 is a cooperative paramagnetic and remains dynamic down to 15 mK and Gd2Ti2O7 enters a unique partially ordered state at {\\sim }1 K.

  6. Static and dynamical spin correlations of the S =1/2 random-bond antiferromagnetic Heisenberg model on the triangular and kagome lattices

    Science.gov (United States)

    Shimokawa, Tokuro; Watanabe, Ken; Kawamura, Hikaru

    2015-10-01

    Inspired by the recent theoretical suggestion that the random-bond S =1 /2 antiferromagnetic Heisenberg model on the triangular and the kagome lattices might exhibit a randomness-induced quantum spin liquid (QSL) behavior when the strength of the randomness exceeds a critical value, and that this "random-singlet state" might be relevant to the QSL behaviors experimentally observed in triangular organic salts κ -(ET) 2Cu2(CN) 3 and EtMe3Sb [Pd(dmit)2] 2 and in kagome herbertsmithite ZnCu3(OH) 6Cl2 , we further investigate the nature of the static and the dynamical spin correlations of these models. We compute the static and the dynamical spin structure factors, S (q ) and S (q ,ω ) , by means of an exact diagonalization method. In both triangular and kagome models, the computed S (q ,ω ) in the random-singlet state depends on the wave vector q only weakly, robustly exhibiting gapless behaviors accompanied by the broad distribution extending to higher energy ω . Especially in the strongly random kagome model, S (q ,ω ) hardly depends on q , and exhibits an almost flat distribution for a wide range of ω , together with a ω =0 peak. These features agree semiquantitatively with the recent neutron-scattering data on a single-crystal herbertsmithite. Furthermore, the computed magnetization curve agrees almost quantitatively with the experimental one recently measured on a single-crystal herbertsmithite. These results suggest that the QSL state observed in herbertsmithite might indeed be the randomness-induced QSL state, i.e., the random-singlet state.

  7. Nonequilibrium antiferromagnetic mixed-spin Ising model.

    Science.gov (United States)

    Godoy, Mauricio; Figueiredo, Wagner

    2002-09-01

    We studied an antiferromagnetic mixed-spin Ising model on the square lattice subject to two competing stochastic processes. The model system consists of two interpenetrating sublattices of spins sigma=1/2 and S=1, and we take only nearest neighbor interactions between pairs of spins. The system is in contact with a heat bath at temperature T, and the exchange of energy with the heat bath occurs via one-spin flip (Glauber dynamics). Besides, the system interacts with an external agency of energy, which supplies energy to it whenever two nearest neighboring spins are simultaneously flipped. By employing Monte Carlo simulations and a dynamical pair approximation, we found the phase diagram for the stationary states of the model in the plane temperature T versus the competition parameter between one- and two-spin flips p. We observed the appearance of three distinct phases, that are separated by continuous transition lines. We also determined the static critical exponents along these lines and we showed that this nonequilibrium model belongs to the universality class of the two-dimensional equilibrium Ising model.

  8. Spin-wave multiple excitations in nanoscale classical Heisenberg antiferromagnets

    Energy Technology Data Exchange (ETDEWEB)

    Hou, Zhuofei [University of Georgia, Athens; Landau, David P [University of Georgia, Athens; Stocks, George Malcolm [ORNL; Brown, G. [Florida State University, Tallahassee

    2015-02-17

    Monte Carlo and spin dynamics techniques have been used to perform large-scale simulations of the dynamic behavior of a nanoscale, classical, Heisenberg antiferromagnet on a simple-cubic lattice with linear sizes L≤ 40 at a temperature below the Neel temperature. In this study, nanoparticles are modeled with completely free boundary conditions, i.e., six free surfaces, and nanofilms are modeled with two free surfaces in the spatial z direction and periodic boundaries parallel to the surfaces in the xy direction, which are compared to the infinite system with periodic boundary conditions. The temporal evolutions of spin configurations were determined numerically from coupled equations of motion for individual spins using a fast spin dynamics algorithm with the fourth-order Suzuki-Trotter decomposition of exponential operators, with initial spin configurations generated by Monte Carlo simulations. The local dynamic structure factor S(q,ω) was calculated from the local space- and time-displaced spin-spin correlation function. Multiple excitation peaks for wave vectors within the first Brillouin zone appear in the spin-wave spectra of the transverse component of dynamic structure factor ST (q,ω) in the nanoscale classical Heisenberg antiferromagnet, which are lacking if periodic boundary conditions are used. With the assumption of q-space spin-wave reflections with broken momentum conservation due to free-surface confinements, we successfully explained those spectra quantitatively in the linear dispersion region. Meanwhile, we also observed two unexpected quantized spin-wave excitation modes in the spatial z direction in nanofilms for ST (q,ω) not expected in bulk systems. In conclusion, the results of this study indicate the presence of unexpected forms of spin-wave excitation behavior that have yet to be observed experimentally but could be directly tested through neutron scattering experiments on nanoscale RbMnF3 particles or

  9. Spin Seebeck effect through antiferromagnetic NiO

    Science.gov (United States)

    Prakash, Arati; Brangham, Jack; Yang, Fengyuan; Heremans, Joseph P.

    2016-07-01

    We report temperature-dependent spin Seebeck measurements on Pt/YIG bilayers and Pt/NiO/YIG trilayers, where YIG (yttrium iron garnet, Y3F e5O12 ) is an insulating ferrimagnet and NiO is an antiferromagnet at low temperatures. The thickness of the NiO layer is varied from 0 to 10 nm. In the Pt/YIG bilayers, the temperature gradient applied to the YIG stimulates dynamic spin injection into the Pt, which generates an inverse spin Hall voltage in the Pt. The presence of a NiO layer dampens the spin injection exponentially with a decay length of 2 ± 0.6 nm at 180 K. The decay length increases with temperature and shows a maximum of 5.5 ± 0.8 nm at 360 K. The temperature dependence of the amplitude of the spin Seebeck signal without NiO shows a broad maximum of 6.5 ± 0.5 μV/K at 20 K. In the presence of NiO, the maximum shifts sharply to higher temperatures, likely correlated to the increase in decay length. This implies that NiO is most transparent to magnon propagation near the paramagnet-antiferromagnet transition. We do not see the enhancement in spin current driven into Pt reported in other papers when 1-2 nm NiO layers are sandwiched between Pt and YIG.

  10. Spin-dynamics simulations of the antiferromagnetic triangular XY model*

    Science.gov (United States)

    Nho, Kwangsik; Landau, D. P.

    2002-03-01

    Using Monte Carlo and spin-dynamics methods, we have simulated the dynamic behavior of the classical, antiferromagnetic XY model on a triangular lattice. The temporal evolutions of spin configurations were obtained by solving numerically the coupled equations of motion for each spin using fourth-order Suzuki-Trotter decompositions of exponential operators. From space-and time-displaced spin-spin correlation functions and their space-time Fourier transforms we obtained the dynamic structure factor S(q,w) for momentum q and frequency w. Below T_c, where long-range order appears in the staggered chirality[1], S(q,w) exhibits very strong and sharp spin-wave peaks in the in-plane-component S^xx. We also observe two-spin-wave peaks at low w and an almost dispersionless domain-wall peak at high w. Above T_c, a weak spin-wave peak persists but the domain-wall peak disappears for all q. We have calculated the dispersion relation and the linewidth of the spin-wave peak in S^xx by fitting the line shape to simple Lorentzians. *Supported by NSF [1] D.H. Lee, J.D. Joannopoulos, J.W. Negele, and D.P. Landau, Phys. Rev. Lett. 52, 433 (1984)

  11. Spin transport through the metallic antiferromagnet FeMn

    Science.gov (United States)

    Saglam, H.; Zhang, W.; Jungfleisch, M. B.; Sklenar, J.; Pearson, J. E.; Ketterson, J. B.; Hoffmann, A.

    2016-10-01

    We investigate spin transport through metallic antiferromagnets using measurements based on spin pumping combined with inverse spin Hall effects in N i80F e20/FeMn /W trilayers. The relatively large magnitude and opposite sign of spin Hall effects in W compared to FeMn enable an unambiguous detection of spin currents transmitted through the entire FeMn layer thickness. Using this approach we can detect two distinctively different spin transport regimes, which we associate with electronic and magnonic spin currents, respectively. The latter can extend to relatively large distances (≈9 nm) and is enhanced when the antiferromagnetic ordering temperature is close to the measurement temperature.

  12. Dynamics of antiferromagnetic skyrmion driven by the spin Hall effect

    Science.gov (United States)

    Jin, Chendong; Song, Chengkun; Wang, Jianbo; Liu, Qingfang

    2016-10-01

    Magnetic skyrmion moved by the spin-Hall effect is promising for the application of the generation racetrack memories. However, the Magnus force causes a deflected motion of skyrmion, which limits its application. Here, we create an antiferromagnetic skyrmion by injecting a spin-polarized pulse in the nanostripe and investigate the spin Hall effect-induced motion of antiferromagnetic skyrmion by micromagnetic simulations. In contrast to ferromagnetic skyrmion, we find that the antiferromagnetic skyrmion has three evident advantages: (i) the minimum driving current density of antiferromagnetic skyrmion is about two orders smaller than the ferromagnetic skyrmion; (ii) the velocity of the antiferromagnetic skyrmion is about 57 times larger than the ferromagnetic skyrmion driven by the same value of current density; (iii) antiferromagnetic skyrmion can be driven by the spin Hall effect without the influence of Magnus force. In addition, antiferromagnetic skyrmion can move around the pinning sites due to its property of topological protection. Our results present the understanding of antiferromagnetic skyrmion motion driven by the spin Hall effect and may also contribute to the development of antiferromagnetic skyrmion-based racetrack memories.

  13. Chiral Magnetic Effect and Anomalous Hall Effect in Antiferromagnetic Insulators with Spin-Orbit Coupling.

    Science.gov (United States)

    Sekine, Akihiko; Nomura, Kentaro

    2016-03-04

    We search for dynamical magnetoelectric phenomena in three-dimensional correlated systems with spin-orbit coupling. We focus on the antiferromagnetic insulator phases where the dynamical axion field is realized by the fluctuation of the antiferromagnetic order parameter. It is shown that the dynamical chiral magnetic effect, an alternating current generation by magnetic fields, emerges due to such time dependences of the order parameter as antiferromagnetic resonance. It is also shown that the anomalous Hall effect arises due to such spatial variations of the order parameter as antiferromagnetic domain walls. Our study indicates that spin excitations in antiferromagnetic insulators with spin-orbit coupling can result in nontrivial charge responses. Moreover, observing the chiral magnetic effect and anomalous Hall effect in our system is equivalent to detecting the dynamical axion field in condensed matter.

  14. Neutron Scattering Studies of Antiferromagnetic Correlations in Cuprates

    OpenAIRE

    Tranquada, John M.

    2005-01-01

    Neutron scattering studies have provided important information about the momentum and energy dependence of magnetic excitations in cuprate superconductors. Of particular interest are the recent indications of a universal magnetic excitation spectrum in hole-doped cuprates. That starting point provides motivation for reviewing the antiferromagnetic state of the parent insulators, and the destruction of the ordered state by hole doping. The nature of spin correlations in stripe-ordered phases i...

  15. Spin Hall magnetoresistance in antiferromagnet/normal metal bilayers

    KAUST Repository

    Manchon, Aurelien

    2017-01-01

    We investigate the emergence of spin Hall magnetoresistance in a magnetic bilayer composed of a normal metal adjacent to an antiferromagnet. Based on a recently derived drift diffusion equation, we show that the resistance of the bilayer depends on the relative angle between the direction transverse to the current flow and the Néel order parameter. While this effect presents striking similarities with the spin Hall magnetoresistance recently reported in ferromagnetic bilayers, its physical origin is attributed to the anisotropic spin relaxation of itinerant spins in the antiferromagnet.

  16. Calculation of generalized spin stiffness constant of strongly correlated doped quantum antiferromagnet on two-dimensional lattice and it's application to effective exchange constant for semi-itinerant systems

    Science.gov (United States)

    Bhattacharjee, Suraka; Chaudhury, Ranjan

    2016-11-01

    The generalized spin stiffness constant for a doped quantum antiferromagnet has been investigated both analytically and numerically as a function of doping concentration at zero temperature, based on the strongly correlated t-J model on two-dimensional square lattice. The nature of the theoretical dependence of the stiffness constant on doping shows a striking similarity with that of the effective exchange constant, obtained from the combination of other theoretical and experimental techniques in the low doping region. This correspondence once again establishes that spin stiffness can very well play the role of an effective exchange constant even in the strongly correlated semi-itinerant systems. Our theoretical plot of the stiffness constant against doping concentration in the whole doping region exhibits the various characteristic features like a possible crossover in the higher doping regions and persistence of short range ordering even for very high doping with the complete vanishing of spin stiffness occurring only close to 100% doping. Our results receive very good support from various other theoretical approaches and also brings out a few limitations of some of them. Our detailed analysis highlights the crucial importance of the study of spin stiffness for the proper understanding of magnetic correlations in a semi-itinerant magnetic system described by the strongly correlated t-J model. Moreover, our basic formalism can also be utilized for determination of the effective exchange constant and magnetic correlations for itinerant magnetic systems, in general in a novel way.

  17. Spin-phonon interaction in antiferromagnetics

    Energy Technology Data Exchange (ETDEWEB)

    Grigorashchuk, I.M.; Nitsovich, V.M.; Tovstyuk, K.D.

    1975-01-01

    The vibrational spectrum and the sound velocity in antiferromagnetics are obtained in the general form in pseudoharmonic approximation with allowance for the anharmonisms of all orders. Starting from experimentally defined dependence of the Debye-Waller factor on the temperature a corollary is put forward that in some antiferromagnetics under the temperature lower than T/subN/ the appearance of the narrow band of paramagnetic states is possible. In antiferromagnetics where the transition metal-dielectric described by the Habbard model is possible this results in the appearance of the additional transition dielectric-metal-dielectric. (auth)

  18. Spin waves in antiferromagnetic FeF2

    DEFF Research Database (Denmark)

    Hutchings, M T; Rainford, B.D.; Guggenheim, H J

    1970-01-01

    Spin-wave dispersion in antiferromagnetic FeF2 has been investigated by inelastic neutron scattering using a chopper time-of-flight spectrometer. The single mode observed has a relatively flat dispersion curve rising from 53 cm-1 at the zone centre to 79 cm-1 at the zone boundary. A spin...

  19. Magnetization damping in noncollinear spin valves with antiferromagnetic interlayer couplings

    Science.gov (United States)

    Chiba, Takahiro; Bauer, Gerrit E. W.; Takahashi, Saburo

    2015-08-01

    We study the magnetic damping in the simplest of synthetic antiferromagnets, i.e., antiferromagnetically exchange-coupled spin valves, in the presence of applied magnetic fields that enforce noncolliear magnetic configurations. We formulate the dynamic exchange of spin currents in a noncollinear texture based on the spin-diffusion theory with quantum mechanical boundary conditions at the ferrromagnet/normal-metal interfaces and derive the Landau-Lifshitz-Gilbert equations coupled by the interlayer static and dynamic exchange interactions. We predict noncollinearity-induced additional damping that is modulated by an applied magnetic field. We compare theoretical results with published experiments.

  20. Spin transfer torque in antiferromagnetic spin valves: From clean to disordered regimes

    KAUST Repository

    Saidaoui, Hamed Ben Mohamed

    2014-05-28

    Current-driven spin torques in metallic spin valves composed of antiferromagnets are theoretically studied using the nonequilibrium Green\\'s function method implemented on a tight-binding model. We focus our attention on G-type and L-type antiferromagnets in both clean and disordered regimes. In such structures, spin torques can either rotate the magnetic order parameter coherently (coherent torque) or compete with the internal antiferromagnetic exchange (exchange torque). We show that, depending on the symmetry of the spin valve, the coherent and exchange torques can either be in the plane, ∝n×(q×n) or out of the plane ∝n×q, where q and n are the directions of the order parameter of the polarizer and the free antiferromagnetic layers, respectively. Although disorder conserves the symmetry of the torques, it strongly reduces the torque magnitude, pointing out the need for momentum conservation to ensure strong spin torque in antiferromagnetic spin valves.

  1. Ultrafast Band Engineering and Transient Spin Currents in Antiferromagnetic Oxides.

    Science.gov (United States)

    Gu, Mingqiang; Rondinelli, James M

    2016-04-29

    We report a dynamic structure and band engineering strategy with experimental protocols to induce indirect-to-direct band gap transitions and coherently oscillating pure spin-currents in three-dimensional antiferromagnets (AFM) using selective phononic excitations. In the Mott insulator LaTiO3, we show that a photo-induced nonequilibrium phonon mode amplitude destroys the spin and orbitally degenerate ground state, reduces the band gap by 160 meV and renormalizes the carrier masses. The time scale of this process is a few hundreds of femtoseconds. Then in the hole-doped correlated metallic titanate, we show how pure spin-currents can be achieved to yield spin-polarizations exceeding those observed in classic semiconductors. Last, we demonstrate the generality of the approach by applying it to the non-orbitally degenerate AFM CaMnO3. These results advance our understanding of electron-lattice interactions in structures out-of-equilibrium and establish a rational framework for designing dynamic phases that may be exploited in ultrafast optoelectronic and optospintronic devices.

  2. Spin injection and absorption in antiferromagnets (Conference Presentation)

    Science.gov (United States)

    Frangou, Lamprini; Merodio, Pablo; Ghosh, Abhijit; Oyarzun, Simon; Auffret, Stephane; Ebels, Ursula; Chshiev, Mair; Bea, Helene; Vila, Laurent; Bailey, William E.; Gambarelli, Serge; Baltz, Vincent

    2016-10-01

    The antiferromagnetic order is expected to have a high potential in next-generation spintronic applications. It is resistant to perturbation by magnetic fields, produces no stray fields, displays ultrafast dynamics and may generate large magneto-transport effects. In spintronic materials, spin currents are key to unravelling spin dependent transport phenomena. Here, spin pumping results from the non-equilibrium magnetization dynamics of a ferromagnetic spin injector, which pumps a spin current into an adjacent spin sink. This spin sink absorbs the current to an extent which depends on its spin-dependent properties. The properties of the spin sink can be recorded either through the changes induced in ferromagnetic damping or through direct electrical means, such as by measuring the inverse spin Hall voltage. In this talk, we will deal with the injection of a spin current in thin antiferromagnetic sinks. Measurements of the spin penetration depths and absorption mechanisms were obtained for polycrystalline Ir20Mn80 and Fe50Mn50 films (Appl. Phys. Lett. 104, 032406 (2014)). More interestingly, spins propagate more efficiently in layers where the magnetic order is fluctuating rather than static. The experimental data were compared to some of the recently developed theories and converted into interfacial spin mixing conductance enhancements. These findings help us progress towards the development of more efficient spin sources, while also providing an alternative method to probe magnetic phase transitions (Phys. Rev. Lett. in press (2016)). This type of alternative method is particularly needed to deal with the case of thin materials with no net magnetic moments, such as thin antiferromagnets.

  3. Spin superconductivity in the frustrated two-dimensional antiferromagnet in the square lattice

    Science.gov (United States)

    Lima, L. S.

    2017-02-01

    We use the SU(2) Schwinger boson formalism to study the spin transport in the two-dimensional S = 1 / 2 frustrated Heisenberg antiferromagnet in a square lattice, considering the second-neighbors interactions in the diagonal. We have obtained a spin superfluid behavior for the spin transport to this system similar to obtained recently to the triangular lattice. We consider an antiferromagnetic inter-chain coupling on the diagonal, J2 > 0 , and the nearest-neighbor coupling antiferromagnetic J1 > 0 . We also have in the critical temperature T0, where the correlation length ξ → 0 , that the system suffers a transition from an ordered ground state to a disordered ground state.

  4. Theory of spin transport in antiferromagnets (Conference Presentation)

    Science.gov (United States)

    Manchon, Aurélien; Saidaoui, Hamed; Akosa, Collins

    2016-10-01

    Antiferromagnets (AF) have long remained an intriguing and exotic state of matter, their application being restricted to enabling interfacial exchange bias in spin-valves. Their role in the expanding field of applied spintronics has been mostly passive and the in-depth investigation of their basic properties considered as fundamental condensed matter physics. A conceptual breakthrough was achieved ten years ago with the proposal that spin transfer torque could be used to electrically control the direction of the order parameter of AF spin valves, henceforth making these materials potential candidates for low energy spin devices. In spite of substantial theoretical efforts and experimental attempts to observe such a torque, the difficulty to independently detect the direction of the AF order parameter has remained a major obstacle. In this talk, I will first introduce the original concept of spin transfer torque in AF spin-valves, demonstrating that it is strongly limited by the spin decoherence and dramatically vanishes in the presence of disorder, leaving little hope to observe this effect experimentally. Then, I will present the newly proposed concept of spin-orbit torque that utilizes bulk or interfacial the spin-orbit coupling in non-centrosymmetric magnets to directly generate a torque on the AF order parameter. This torque, being local, is much more robust against impurities, as will be demonstrated for the specific case of interfacial Rashba spin-orbit coupling. Finally, I will discuss about spin motive force and torques in antiferromagnetic textures, intriguing effects that remained to be experimentally observed.

  5. Distinct spin liquids and their transitions in spin-1/2 XXZ kagome antiferromagnets.

    Science.gov (United States)

    He, Yin-Chen; Chen, Yan

    2015-01-23

    By using the density matrix renormalization group approach, we study spin-liquid phases of spin-1/2 XXZ kagome antiferromagnets. We find that the emergence of the spin-liquid phase is independent of the anisotropy of the XXZ interaction. In particular, the two extreme limits-the Ising (a strong S^{z} interaction) and the XY (zero S^{z} interaction)-host the same spin-liquid phases as the isotropic Heisenberg model. Both a time-reversal-invariant spin liquid and a chiral spin liquid with spontaneous time-reversal symmetry breaking are obtained. We show that they evolve continuously into each other by tuning the second- and the third-neighbor interactions. And last, we discuss possible implications of our results for the nature of spin liquid in nearest-neighbor XXZ kagome antiferromagnets, including the nearest-neighbor spin-1/2 kagome antiferromagnetic Heisenberg model.

  6. Domain-wall spin dynamics in kagome antiferromagnets.

    Science.gov (United States)

    Lhotel, E; Simonet, V; Ortloff, J; Canals, B; Paulsen, C; Suard, E; Hansen, T; Price, D J; Wood, P T; Powell, A K; Ballou, R

    2011-12-16

    We report magnetization and neutron scattering measurements down to 60 mK on a new family of Fe based kagome antiferromagnets, in which a strong local spin anisotropy combined with a low exchange path network connectivity lead to domain walls intersecting the kagome planes through strings of free spins. These produce unfamiliar slow spin dynamics in the ordered phase, evolving from exchange-released spin flips towards a cooperative behavior on decreasing the temperature, probably due to the onset of long-range dipolar interaction. A domain structure of independent magnetic grains is obtained that could be generic to other frustrated magnets.

  7. Spin Hall effects in metallic antiferromagnets – perspectives for future spin-orbitronics

    Directory of Open Access Journals (Sweden)

    Joseph Sklenar

    2016-05-01

    Full Text Available We investigate angular dependent spin-orbit torques from the spin Hall effect in a metallic antiferromagnet using the spin-torque ferromagnetic resonance technique. The large spin Hall effect exists in PtMn, a prototypical CuAu-I-type metallic antiferromagnet. By applying epitaxial growth, we previously reported an appreciable difference in spin-orbit torques for c- and a-axis orientated samples, implying anisotropic effects in magnetically ordered materials. In this work we demonstrate through bipolar-magnetic-field experiments a small but noticeable asymmetric behavior in the spin-transfer-torque that appears as a hysteresis effect. We also suggest that metallic antiferromagnets may be good candidates for the investigation of various unidirectional effects related to novel spin-orbitronics phenomena.

  8. The Berezinskii-Kosterlitz-Thouless transition and correlations in the XY kagome antiferromagnet

    CERN Document Server

    Cherepanov, V B; Podivilov, E V

    2001-01-01

    The problem of the Berezinskii-Kosterlitz-Thouless transition in the highly frustrated XY antiferromagnetic is solved. The transition temperature is found. It is shown that the spin correlation function exponentially decays with distance even in the low-temperature phase, in contrast to the order parameter correlation function, which decays algebraically with distance

  9. Ultrafast spin dynamics and switching via spin transfer torque in antiferromagnets with weak ferromagnetism

    Science.gov (United States)

    Kim, Tae Heon; Grünberg, Peter; Han, Song Hee; Cho, Beongki

    2016-01-01

    The spin-torque driven dynamics of antiferromagnets with Dzyaloshinskii-Moriya interaction (DMI) were investigated based on the Landau-Lifshitz-Gilbert-Slonczewski equation with antiferromagnetic and ferromagnetic order parameters (l and m, respectively). We demonstrate that antiferromagnets including DMI can be described by a 2-dimensional pendulum model of l. Because m is coupled with l, together with DMI and exchange energy, close examination of m provides fundamental understanding of its dynamics in linear and nonlinear regimes. Furthermore, we discuss magnetization reversal as a function of DMI and anisotropy energy induced by a spin current pulse. PMID:27713522

  10. Ultrafast spin dynamics and switching via spin transfer torque in antiferromagnets with weak ferromagnetism

    Science.gov (United States)

    Kim, Tae Heon; Grünberg, Peter; Han, Song Hee; Cho, Beongki

    2016-10-01

    The spin-torque driven dynamics of antiferromagnets with Dzyaloshinskii-Moriya interaction (DMI) were investigated based on the Landau-Lifshitz-Gilbert-Slonczewski equation with antiferromagnetic and ferromagnetic order parameters (l and m, respectively). We demonstrate that antiferromagnets including DMI can be described by a 2-dimensional pendulum model of l. Because m is coupled with l, together with DMI and exchange energy, close examination of m provides fundamental understanding of its dynamics in linear and nonlinear regimes. Furthermore, we discuss magnetization reversal as a function of DMI and anisotropy energy induced by a spin current pulse.

  11. Persistent spin excitations in doped antiferromagnets revealed by resonant inelastic light scattering

    Science.gov (United States)

    Jia, C. J.; Nowadnick, E. A.; Wohlfeld, K.; Kung, Y. F.; Chen, C.-C.; Johnston, S.; Tohyama, T.; Moritz, B.; Devereaux, T. P.

    2014-02-01

    How coherent quasiparticles emerge by doping quantum antiferromagnets is a key question in correlated electron systems, whose resolution is needed to elucidate the phase diagram of copper oxides. Recent resonant inelastic X-ray scattering (RIXS) experiments in hole-doped cuprates have purported to measure high-energy collective spin excitations that persist well into the overdoped regime and bear a striking resemblance to those found in the parent compound, challenging the perception that spin excitations should weaken with doping and have a diminishing effect on superconductivity. Here we show that RIXS at the Cu L3-edge indeed provides access to the spin dynamical structure factor once one considers the full influence of light polarization. Further we demonstrate that high-energy spin excitations do not correlate with the doping dependence of Tc, while low-energy excitations depend sensitively on doping and show ferromagnetic correlations. This suggests that high-energy spin excitations are marginal to pairing in cuprate superconductors.

  12. Theory of the spin Seebeck effect in antiferromagnets

    Science.gov (United States)

    Rezende, S. M.; Rodríguez-Suárez, R. L.; Azevedo, A.

    2016-01-01

    The spin Seebeck effect (SSE) consists in the generation of a spin current by a temperature gradient applied in a magnetic film. The SSE is usually detected by an electric voltage generated in a metallic layer in contact with the magnetic film resulting from the conversion of the spin current into charge current by means of the inverse spin Hall effect. The SSE has been widely studied in bilayers made of the insulating ferrimagnet yttrium iron garnet (YIG) and metals with large spin-orbit coupling such as platinum. Recently the SSE has been observed in bilayers made of the antiferromagnet Mn F2 and Pt, revealing dependences of the SSE voltage on temperature and field very different from the ones observed in YIG/Pt. Here we present a theory for the SSE in structures with an antiferromagnetic insulator (AFI) in contact with a normal metal (NM) that relies on the bulk magnon spin current created by the temperature gradient across the thickness of the AFI/NM bilayer. The theory explains quite well the measured dependences of the SSE voltage on the sample temperature and on the applied magnetic field in Mn F2/Pt .

  13. Spin transport of the frustrated integer spin S antiferromagnetic Heisenberg chain

    Energy Technology Data Exchange (ETDEWEB)

    Lima, Leonardo S., E-mail: lslima@infis.ufu.br [Instituto de Física, Universidade Federal de Uberlândia, UFU, CEP:38700-128, Patos de Minas, MG (Brazil); Departamento de Física, ICEx, Universidade Federal de Minas Gerais, CEP:31270-901, Belo Horizonte, MG (Brazil)

    2014-03-15

    We study the effect of the nearest-neighbor (nn) and next-nearest-neighbor (nnn) interactions on spin transport in the quantum integer spin one-dimensional isotropic antiferromagnetic Heisenberg model. The Kubo formalism of the linear response theory is used to calculate the spin conductivity. We obtain the regular part of the spin conductivity, σ{sup reg}(ω), as function of the frequency at T=0 and obtain a strong effect of the (nnn) interaction on magnon transport.

  14. Long range anti-ferromagnetic spin model for prebiotic evolution

    Energy Technology Data Exchange (ETDEWEB)

    Nokura, Kazuo [Shonan Institute of Technology, Fujisawa 251-8511 (Japan)

    2003-11-28

    I propose and discuss a fitness function for one-dimensional binary monomer sequences of macromolecules for prebiotic evolution. The fitness function is defined by the free energy of polymers in the high temperature random coil phase. With repulsive interactions among the same kind of monomers, the free energy in the high temperature limit becomes the energy function of the one-dimensional long range anti-ferromagnetic spin model, which is shown to have a dynamical phase transition and glassy states.

  15. Terahertz-Driven Nonlinear Spin Response of Antiferromagnetic Nickel Oxide

    Science.gov (United States)

    Baierl, S.; Mentink, J. H.; Hohenleutner, M.; Braun, L.; Do, T.-M.; Lange, C.; Sell, A.; Fiebig, M.; Woltersdorf, G.; Kampfrath, T.; Huber, R.

    2016-11-01

    Terahertz magnetic fields with amplitudes of up to 0.4 Tesla drive magnon resonances in nickel oxide while the induced dynamics is recorded by femtosecond magneto-optical probing. We observe distinct spin-mediated optical nonlinearities, including oscillations at the second harmonic of the 1 THz magnon mode. The latter originate from coherent dynamics of the longitudinal component of the antiferromagnetic order parameter, which are probed by magneto-optical effects of second order in the spin deflection. These observations allow us to dynamically disentangle electronic from lattice-related contributions to magnetic linear birefringence and dichroism—information so far only accessible by ultrafast THz spin control. The nonlinearities discussed here foreshadow physics that will become essential in future subcycle spin switching.

  16. Resonant spin tunneling in small antiferromagnetic particles

    Science.gov (United States)

    Luis, F.; del Barco, E.; Hernández, J. M.; Remiro, E.; Bartolomé, J.; Tejada, J.

    1999-05-01

    The paper reports a detailed experimental study on magnetic relaxation of natural horse-spleen ferritin. ac susceptibility measurements performed on three samples of different concentration show that dipole-dipole interactions between uncompensated moments play no significant role. Furthermore, the distribution of relaxation times in these samples has been obtained from a scaling of experimental χ'' data, obtained at different frequencies. The average uncompensated magnetic moment per protein is compatible with a disordered arrangement of atomic spins throughout the core, rather than with surface disorder. The observed field dependence of the blocking temperature suggests that magnetic relaxation is faster at zero field than at intermediate field values. This is confirmed by the fact that the magnetic viscosity peaks at zero field, too. Using the distribution of relaxation times obtained independently, we show that these results cannot be explained in terms of classical relaxation theory. The most plausible explanation of these results is the existence, near zero field, of resonant magnetic tunneling between magnetic states of opposite orientation, which are thermally populated.

  17. Striped spin liquid crystal ground state instability of kagome antiferromagnets.

    Science.gov (United States)

    Clark, Bryan K; Kinder, Jesse M; Neuscamman, Eric; Chan, Garnet Kin-Lic; Lawler, Michael J

    2013-11-01

    The Dirac spin liquid ground state of the spin 1/2 Heisenberg kagome antiferromagnet has potential instabilities. This has been suggested as the reason why it does not emerge as the ground state in large-scale numerical calculations. However, previous attempts to observe these instabilities have failed. We report on the discovery of a projected BCS state with lower energy than the projected Dirac spin liquid state which provides new insight into the stability of the ground state of the kagome antiferromagnet. The new state has three remarkable features. First, it breaks spatial symmetry in an unusual way that may leave spinons deconfined along one direction. Second, it breaks the U(1) gauge symmetry down to Z(2). Third, it has the spatial symmetry of a previously proposed "monopole" suggesting that it is an instability of the Dirac spin liquid. The state described herein also shares a remarkable similarity to the distortion of the kagome lattice observed at low Zn concentrations in Zn-paratacamite and in recently grown single crystals of volborthite suggesting it may already be realized in these materials.

  18. Quenching the haldane gap in spin-1 Heisenberg antiferromagnets.

    Science.gov (United States)

    Wierschem, Keola; Sengupta, Pinaki

    2014-06-20

    We consider a quasi-one-dimensional system of spin-1 Heisenberg antiferromagnetic chains in two-dimensional and three-dimensional hypercubic lattices with interchain coupling J and uniaxial single-ion anisotropy D. Using large-scale numerical simulations, we map out the J-D phase diagram and investigate the low-lying excitations of the Haldane phase in the J≪1 limit. We also provide direct evidence that the Haldane phase remains a nontrivial symmetry-protected topological state for small but finite J.

  19. Antiferromagnetic exchange and spin-fluctuation pairing in cuprate superconductors

    Science.gov (United States)

    Plakida, Nikolay M.

    2006-01-01

    A microscopic theory of superconductivity is formulated within an effective p-d Hubbard model for a CuO2 plane. By applying the Mori-type projection technique, the Dyson equation is derived for the Green functions in terms of Hubbard operators. The antiferromagnetic exchange caused by interband hopping results in pairing of all carries in the conduction subband and high Tc proportional to the Fermi energy. Kinematic interaction in intraband hopping is responsible for the conventional spin-fluctuation pairing. Numerical solution of the gap equation proves the d-wave gap symmetry and defines Tc doping dependence. Oxygen isotope shift and pressure dependence of Tc are also discussed.

  20. Correlation Functions and Spin

    CERN Document Server

    Tyc, T

    2000-01-01

    The k-electron correlation function of a free chaotic electron beam is derived with the spin degree of freedom taken into account. It is shown that it can be expressed with the help of correlation functions for a polarized electron beam of all orders up to k and the degree of spin polarization. The form of the correlation function suggests that if the electron beam is not highly polarized, observing multi-particle correlations should be difficult. The result can be applied also to chaotic photon beams, the degree of spin polarization being replaced by the degree of polarization.

  1. Correlations between Kondo clouds in nearly antiferromagnetic Kondo lattices

    Energy Technology Data Exchange (ETDEWEB)

    Kiselev, M.N. E-mail: kiselev@physik.uni-wuerzburg.de; Kikoin, K.A

    2004-05-01

    We discuss a novel fluctuational mechanism explaining the physics of nearly antiferromagnetic Kondo lattices (KL). The effective action for KL model is expressed in terms of Bose operators responsible for paramagnetic excitations and semi-bosonic fields describing the dynamic Kondo clouds created by conduction electrons around local spin. The gauge invariant resonance valence bond theory of interacting Kondo clouds describes the spin liquid with strong critical fluctuations imitating itinerant fluctuation magnetism of Moriya type.

  2. Spin-dynamics simulations of the triangular antiferromagnetic XY model*

    Science.gov (United States)

    Nho, Kwangsik; Landau, D. P.

    2003-03-01

    Using Monte Carlo and spin-dynamics methods, we have studied the dynamic behavior of the classical, antiferromagnetic XY model on a triangular lattice. The temporal evolutions of spin configurations were obtained by solving numerically the coupled equations of motion for each spin using fourth-order Suzuki-Trotter decompositions of exponential operators. We calculated the dynamic structure factor S(q,w) for momentum q and frequency w. Below T_KT (Kosteritz-Thouless transition), both the in-plane (S^xx) and out-of-plane (S^zz) components exhibit very strong and sharp spin-wave peaks. Well above T_KT, S^xx and S^zz apparently display a central peak, and spin-wave signatures are still seen in S^zz. In addition, we also observed an almost dispersionless domain-wall peak at high w below Tc (Ising transition), where long-range order appears in the staggered chirality[1]. We found that our results demonstrate the consistency of the dynamic finite-size scaling theory for the characteristic frequency wm and S(q,w). *Supported by NSF [1] D.H. Lee, J.D. Joannopoulos, J.W. Negele, and D.P. Landau, Phys. Rev. Lett. 52, 433 (1984)

  3. Spin-Transfer-Torques at a Ferromagnet/Antiferromagnet Interface

    Science.gov (United States)

    Tsoi, Maxim

    2009-03-01

    Spintronics in ferromagnetic systems is built on a complementary set of phenomena in which the magnetic configuration of the system influences its transport properties and vice versa. Giant magnetoresistance (GMR) [1] and spin- transfer-torque (STT) [2] phenomena are typical examples of such interconnections. Recently, MacDonald and co-workers [3] predicted that corresponding effects ought to occur in systems where ferromagnetic (F) components are replaced by antiferromagnets (AFM). I will present our experimental search for these new AFM effects which may potentially lead to a new all-antiferromagnetic spintronics where antiferromagnets are used in place of ferromagnets. In particular I will focus on our experiments with exchange-biased spin valves [4] where extreme current densities were found to affect the exchange bias at F/AFM interface [5-7]. As exchange bias is known to be associated with interfacial AFM magnetic moments, our observation can be taken as the first evidence of STT effect in AFM materials. [4pt] [1] M. N. Baibich et al., Phys. Rev. Lett. 61, 2472 (1988); G. Binasch et al., Phys. Rev. B 39, 4828 (1989). [0pt] [2] J. C. Slonczewski, J. Magn. Magn. Mater. 159, L1 (1996); L. Berger, J. Appl. Phys. 81, 4880 (1997); M. Tsoi et al., Phys. Rev. Lett. 80, 4281 (1998). [0pt] [3] A. S. N'uñez et al., Phys. Rev. B 73, 214426 (2006); [0pt] [4] Z. Wei et al., Phys. Rev. Lett. 98, 116603 (2007). [0pt] [5] S. Urazhdin and N. Anthony, Phys. Rev. Lett. 99, 046602 (2007). [0pt] [6] X-L.Tang et al., Appl. Phys. Lett. 91, 122504 (2007). [0pt] [7] N. V. Dai et al., Phys. Rev. B77, 132406 (2008).

  4. Numerical study of the spin-flop transition in anisotropic spin-1/2 antiferromagnets

    NARCIS (Netherlands)

    Yunoki, S

    2002-01-01

    Magnetization processes of the spin-1/2 antiferromagnetic XXZ model in two and three spatial dimensions are studied using a quantum Monte Carlo method based on stochastic series expansions. A recently developed operator-loop algorithm enables us to show clear evidence of a first-order phase transiti

  5. Spin dynamics in charge doped antiferromagnets : a Li-7 NMR study in Ni1-xLixO

    NARCIS (Netherlands)

    Tedoldi, F; Marini, S; Corti, M

    1997-01-01

    The effects of heterovalent substitutions causing itinerant holes in strongly correlated 3d electron systems are studied by means of Li-7 NMR in lithium-doped antiferromagnetic NiO. The spin-lattice relaxation rates, driven by the fluctuation of Ni2+ (S = 1) ions, in the temperature range 10 K

  6. Higher-spin correlators

    CERN Document Server

    Alday, Luis F

    2013-01-01

    We analyze the properly normalized three-point correlator of two protected scalar operators and one higher spin twist-two operator in N=4 super Yang-Mills, in the limit of large spin j. The relevant structure constant can be extracted from the OPE of the four-point correlator of protected scalar operators. We show that crossing symmetry of the four point correlator plus a judicious guess for the perturbative structure of the three-point correlator, allow to make a prediction for the structure constant at all loops in perturbation theory, up to terms that remain finite as the spin becomes large. Furthermore, the expression for the structure constant allows to propose an expression for the all loops four-point correlator G(u,v), in the limit u,v -> 0. Our predictions are in perfect agreement with the large j expansion of results available in the literature.

  7. Spin-flop states in a synthetic antiferromagnet and variations of unidirectional anisotropy in FeMn-based spin valves

    Science.gov (United States)

    Milyaev, M. A.; Naumova, L. I.; Chernyshova, T. A.; Proglyado, V. V.; Kulesh, N. A.; Patrakov, E. I.; Kamenskii, I. Yu.; Ustinov, V. V.

    2016-12-01

    Spin valves with a synthetic antiferromagnet have been prepared by magnetron sputtering. Regularities of the formation of single- and two-phase spin-flop states in the synthetic antiferromagnet have been studied using magnetoresistance measurements and imaging the magnetic structure. A thermomagnetic treatment of spin valve in a field that corresponds to the single-phase spin-flop state of synthetic antiferromagnet was shown to allow us to obtain a magnetically sensitive material characterized by hysteresis-free field dependence of the magnetoresistance.

  8. Anisotropic spin model of strong spin-orbit-coupled triangular antiferromagnets

    Science.gov (United States)

    Li, Yao-Dong; Wang, Xiaoqun; Chen, Gang

    2016-07-01

    Motivated by the recent experimental progress on the strong spin-orbit-coupled rare-earth triangular antiferromagnet, we analyze the highly anisotropic spin model that describes the interaction between the spin-orbit-entangled Kramers' doublet local moments on the triangular lattice. We apply the Luttinger-Tisza method, the classical Monte Carlo simulation, and the self-consistent spin wave theory to analyze the anisotropic spin Hamiltonian. The classical phase diagram includes the 120∘ state and two distinct stripe-ordered phases. The frustration is very strong and significantly suppresses the ordering temperature in the regimes close to the phase boundary between two ordered phases. Going beyond the semiclassical analysis, we include the quantum fluctuations of the spin moments within a self-consistent Dyson-Maleev spin-wave treatment. We find that the strong quantum fluctuations melt the magnetic order in the frustrated regions. We explore the magnetic excitations in the three different ordered phases as well as in strong magnetic fields. Our results provide a guidance for the future theoretical study of the generic model and are broadly relevant for strong spin-orbit-coupled triangular antiferromagnets such as YbMgGaO4, RCd3P3 , RZn3P3 , RCd3As3 , RZn3As3 , and R2O2CO3 .

  9. Antiferromagnetic spin correlations between corner-shared [FeO5]7- and [FeO6]9- units, in the novel iron-based compound: BaYFeO4.

    Science.gov (United States)

    Wrobel, Friederike; Kemei, Moureen C; Derakhshan, Shahab

    2013-03-04

    A novel quaternary compound in the Ba-Y-Fe-O phase diagram was synthesized by solid-state reaction and its crystal structure was characterized using powder X-ray diffraction. The crystal structure of BaYFeO4 consists of a unique arrangement of Fe(3+) magnetic ions, which is based on alternate corner-shared units of [FeO5](7-) square pyramids and [FeO6](9-) octahedra. This results in the formation of stairwise channels of FeO polyhedra along the b crystallographic axis. The structure is described in an orthorhombic crystal system in the space group Pnma with lattice parameters a = 13.14455(1) Å, b = 5.694960(5) Å, and c = 10.247630(9) Å. The temperature-dependent magnetic susceptibility data reveal two antiferromagnetic (AFM) transitions at 33 and 48 K. An upturn in the magnetic susceptibility data above these transitions is observed, which does not reach its maximum even at 390 K. The field-dependent magnetization data at both 2 and 300 K show a nearly linear dependence and do not exhibit significant hysteresis. Heat capacity measurements between 2 and 200 K reveal only a broad anomaly without any indication of long-range ordering. The latter data set is not in good agreement with the magnetic susceptibility data, which makes it difficult to exactly determine the magnetic ground state of BaYFeO4. Accordingly, a temperature-dependent neutron diffraction study is in order, which will enable resolving this issue. The theoretical study of the relative strengths of magnetic exchange interactions along various possible pathways, using extended Hückel spin dimer analysis, shows that only interactions between square pyramidal and octahedral centers are significant, and among them, the intrachannel correlations are stronger than interchannel interactions. This is the first physical property study in such a magnetic ion substructure.

  10. Evolution of spin excitations in a gapped antiferromagnet from the quantum to the high-temperature limit

    DEFF Research Database (Denmark)

    Kenzelmann, M.; Cowley, R.A.; Buyers, W.J.L.

    2002-01-01

    is in agreement with quantum Monte Carlo calculations for the spin-1 chain. xi is also consistent with the single mode approximation, suggesting that the excitations are short-lived single particle excitations. Below T=12 K where three-dimensional spin correlations are important, xi is shorter than predicted......We have mapped from the quantum to the classical limit the spin excitation spectrum of the antiferromagnetic spin-1 Heisenberg chain system CsNiCl3 in its paramagnetic phase from T=5 to 200 K. Neutron scattering shows that the excitations are resonant and dispersive up to at least T=70 Ksimilar...

  11. Quantum entanglement in trimer spin-1/2 Heisenberg chains with antiferromagnetic coupling

    CERN Document Server

    Del Cima, O M; da Silva, S L L

    2015-01-01

    The quantum entanglement measure is determined, for the first time, for antiferromagnetic trimer spin-1/2 Heisenberg chains. The physical quantity proposed to measure the entanglement is the distance between states by adopting the Hilbert-Schmidt norm. The method is applied to the new magnetic Cu(II) trimer system, 2b.3CuCl_2.2H_2O, and to the trinuclear Cu(II) halide salt, (3MAP)_2Cu_2Cl_8. The decoherence temperature, above which the entanglement is suppressed, is determined for the both systems. A correlation among their decoherence temperatures and their respective exchange coupling constants is established.

  12. Spin freezing in the geometrically frustrated pyrochlore antiferromagnet Tb2Mo2O7

    DEFF Research Database (Denmark)

    Gaulin, B.D.; Reimers, J.N.; Mason, T.E.

    1992-01-01

    The magnetic metal ions in the cubic pyrochlore Tb2Mo2O7 form an infinite three-dimensional network of corner-sharing tetrahedra with a very high potential for frustration in the presence of antiferromagnetism. We have performed neutron scattering measurements which show short-range spatial...... correlations that develop continuously with decreasing temperature, while the characteristic time scale for the fluctuating moments decreases dramatically below T(f) is similar to 25 K. Therefore, this pure material, which possesses frustration that is purely geometrical in origin, displays a spin-glass state...

  13. Topological Phases of the Spin-1/2 Ferromagnetic--Antiferromagnetic Alternating Heisenberg Chain with Frustrated Next-Nearest-Neighbour Interaction

    Science.gov (United States)

    Hida, Kazuo; Takano, Ken'ichi; Suzuki, Hidenori

    2013-06-01

    The spin-1/2 ferromagnetic--antiferromagnetic alternating Heisenberg chain with ferromagnetic next-nearest-neighbour (NNN) interaction is investigated. The ground state is the Haldane phase for weak NNN interaction, and is the ferromagnetic phase for weak antiferromagnetic interaction. We find a series of topologically distinct spin-gap phases with various magnitudes of edge spins for strong NNN interaction. The phase boundaries between these phases are determined on the basis of the DMRG calculation with additional spins that compensate the edge spins. It is found that each of the exact solutions with short-range antiferromagnetic correlation on the ferromagnetic--nonmagnetic phase boundary is representative of each spin gap phase.

  14. Spin liquid nature in the Heisenberg J1-J2 triangular antiferromagnet

    Science.gov (United States)

    Iqbal, Yasir; Hu, Wen-Jun; Thomale, Ronny; Poilblanc, Didier; Becca, Federico

    2016-04-01

    We investigate the spin-1/2 Heisenberg model on the triangular lattice in the presence of nearest-neighbor J1 and next-nearest-neighbor J2 antiferromagnetic couplings. Motivated by recent findings from density-matrix renormalization group (DMRG) claiming the existence of a gapped spin liquid with signatures of spontaneously broken lattice point group symmetry [Zhu and White, Phys. Rev. B 92, 041105 (2015), 10.1103/PhysRevB.92.041105 and Hu, Gong, Zhu, and Sheng, Phys. Rev. B 92, 140403 (2015), 10.1103/PhysRevB.92.140403], we employ the variational Monte Carlo (VMC) approach to analyze the model from an alternative perspective that considers both magnetically ordered and paramagnetic trial states. We find a quantum paramagnet in the regime 0.08 ≲J2/J1≲0.16 , framed by 120∘ coplanar (stripe collinear) antiferromagnetic order for smaller (larger) J2/J1 . By considering the optimization of spin-liquid wave functions of a different gauge group and lattice point group content as derived from Abrikosov mean-field theory, we obtain the gapless U(1 ) Dirac spin liquid as the energetically most preferable state in comparison to all symmetric or nematic gapped Z2 spin liquids so far advocated by DMRG. Moreover, by the application of few Lanczos iterations, we find the energy to be the same as the DMRG result within error bars. To further resolve the intriguing disagreement between VMC and DMRG, we complement our methodological approach by the pseudofermion functional renormalization group (PFFRG) to compare the spin structure factors for the paramagnetic regime calculated by VMC, DMRG, and PFFRG. This model promises to be an ideal test bed for future numerical refinements in tracking the long-range correlations in frustrated magnets.

  15. Spin-S kagome quantum antiferromagnets in a field with tensor networks

    Science.gov (United States)

    Picot, Thibaut; Ziegler, Marc; Orús, Román; Poilblanc, Didier

    2016-02-01

    Spin-S Heisenberg quantum antiferromagnets on the kagome lattice offer, when placed in a magnetic field, a fantastic playground to observe exotic phases of matter with (magnetic analogs of) superfluid, charge, bond, or nematic orders, or a coexistence of several of the latter. In this context, we have obtained the (zero-temperature) phase diagrams up to S =2 directly in the thermodynamic limit owing to infinite projected entangled pair states, a tensor network numerical tool. We find incompressible phases characterized by a magnetization plateau versus field and stabilized by spontaneous breaking of point group or lattice translation symmetry(ies). The nature of such phases may be semiclassical, as the plateaus at the 1/3th ,(1-2/9S)th, and (1-1/9S)th of the saturated magnetization (the latter followed by a macroscopic magnetization jump), or fully quantum as the spin-1/2 1/9 plateau exhibiting a coexistence of charge and bond orders. Upon restoration of the spin rotation U (1 ) symmetry, a finite compressibility appears, although lattice symmetry breaking persists. For integer spin values we also identify spin gapped phases at low enough fields, such as the S =2 (topologically trivial) spin liquid with no symmetry breaking, neither spin nor lattice.

  16. Quantum Monte Carlo study of the itinerant-localized model of strongly correlated electrons: Spin-spin correlation functions

    OpenAIRE

    Ivantsov, Ilya; Ferraz, Alvaro; Kochetov, Evgenii

    2016-01-01

    We perform quantum Monte Carlo simulations of the itinerant-localized periodic Kondo-Heisenberg model for the underdoped cuprates to calculate the associated spin correlation functions. The strong electron correlations are shown to play a key role in the abrupt destruction of the quasi long-range antiferromagnetic order in the lightly doped regime.

  17. Quantum Monte Carlo study of the itinerant-localized model of strongly correlated electrons: Spin-spin correlation functions

    Science.gov (United States)

    Ivantsov, Ilya; Ferraz, Alvaro; Kochetov, Evgenii

    2016-12-01

    We perform quantum Monte Carlo simulations of the itinerant-localized periodic Kondo-Heisenberg model for the underdoped cuprates to calculate the associated spin correlation functions. The strong electron correlations are shown to play a key role in the abrupt destruction of the quasi-long-range antiferromagnetic order in the lightly doped regime.

  18. Spin torque antiferromagnetic nanooscillator in the presence of magnetic noise

    Directory of Open Access Journals (Sweden)

    H. Gomonay

    2012-12-01

    Full Text Available Spin-torque effects in antiferromagnetic (AFM materials are of great interest due to the possible applications as high-speed spintronic devices. In the present paper we analyze the statistical properties of the current-driven AFM nanooscillator that result from the white Gaussian noise of magnetic nature. According to the peculiarities of deterministic dynamics, we derive the Langevin and Fokker-Planck equations in the energy representation of two normal modes. We find the stationary distribution function in the subcritical and overcritical regimes and calculate the current dependence of the average energy, energy fluctuation and their ratio (quality factor. The noncritical mode shows the Boltzmann statistics with the current-dependent effective temperature in the whole range of the current values. The effective temperature of the other, i.e., soft, mode critically depends on the current in the subcritical region. Distribution function of the soft mode follows the Gaussian law above the generation threshold. In the overcritical regime, the total average energy and the quality factor grow with the current value. This raises the AFM nanooscillators to the promising candidates for active spintronic components.

  19. Spin-orbit torque in two-dimensional antiferromagnetic topological insulators

    KAUST Repository

    Ghosh, S.

    2017-01-24

    We investigate spin transport in two-dimensional ferromagnetic (FTI) and antiferromagnetic (AFTI) topological insulators. In the presence of an in-plane magnetization AFTI supports zero energy modes, which enables topologically protected edge conduction at low energy. We address the nature of current-driven spin torque in these structures and study the impact of spin-independent disorder. Interestingly, upon strong disorder the spin torque develops an antidamping component (i.e., even upon magnetization reversal) along the edges, which could enable current-driven manipulation of the antiferromagnetic order parameter. This antidamping torque decreases when increasing the system size and when the system enters the trivial insulator regime.

  20. Persistent nonequilibrium dynamics of the thermal energies in the spin and phonon systems of an antiferromagnet.

    Science.gov (United States)

    von Reppert, A; Pudell, J; Koc, A; Reinhardt, M; Leitenberger, W; Dumesnil, K; Zamponi, F; Bargheer, M

    2016-09-01

    We present a temperature and fluence dependent Ultrafast X-Ray Diffraction study of a laser-heated antiferromagnetic dysprosium thin film. The loss of antiferromagnetic order is evidenced by a pronounced lattice contraction. We devise a method to determine the energy flow between the phonon and spin system from calibrated Bragg peak positions in thermal equilibrium. Reestablishing the magnetic order is much slower than the cooling of the lattice, especially around the Néel temperature. Despite the pronounced magnetostriction, the transfer of energy from the spin system to the phonons in Dy is slow after the spin-order is lost.

  1. Persistent nonequilibrium dynamics of the thermal energies in the spin and phonon systems of an antiferromagnet

    Directory of Open Access Journals (Sweden)

    A. von Reppert

    2016-09-01

    Full Text Available We present a temperature and fluence dependent Ultrafast X-Ray Diffraction study of a laser-heated antiferromagnetic dysprosium thin film. The loss of antiferromagnetic order is evidenced by a pronounced lattice contraction. We devise a method to determine the energy flow between the phonon and spin system from calibrated Bragg peak positions in thermal equilibrium. Reestablishing the magnetic order is much slower than the cooling of the lattice, especially around the Néel temperature. Despite the pronounced magnetostriction, the transfer of energy from the spin system to the phonons in Dy is slow after the spin-order is lost.

  2. Antiferromagnetic Heisenberg Spin Chain of a Few Cold Atoms in a One-Dimensional Trap.

    Science.gov (United States)

    Murmann, S; Deuretzbacher, F; Zürn, G; Bjerlin, J; Reimann, S M; Santos, L; Lompe, T; Jochim, S

    2015-11-20

    We report on the deterministic preparation of antiferromagnetic Heisenberg spin chains consisting of up to four fermionic atoms in a one-dimensional trap. These chains are stabilized by strong repulsive interactions between the two spin components without the need for an external periodic potential. We independently characterize the spin configuration of the chains by measuring the spin orientation of the outermost particle in the trap and by projecting the spatial wave function of one spin component on single-particle trap levels. Our results are in good agreement with a spin-chain model for fermionized particles and with numerically exact diagonalizations of the full few-fermion system.

  3. Painlevé transcendent describes quantum correlation function of the XXZ antiferromagnet away from the free-fermion point

    CERN Document Server

    Essler, F H L; Its, A R; Korepin, V E; Essler, Fabian H L; Frahm, Holger; Its, Alexander R; Korepin, Vladimir E

    1996-01-01

    We consider quantum correlation functions of the antiferromagnetic spin-\\frac{1}{2} Heisenberg XXZ spin chain in a magnetic field. We show that for a magnetic field close to the critical field h_c (for the critical magnetic field the ground state is ferromagnetic) certain correlation functions can be expressed in terms of the solution of the Painlev\\'e V transcendent. This establishes a relation between solutions of Painlev\\'e differential equations and quantum correlation functions in models of {\\sl interacting} fermions. Painlev\\'e transcendents were known to describe correlation functions in models with free fermionic spectra.

  4. Evidence for a gapped spin-liquid ground state in a kagome Heisenberg antiferromagnet.

    Science.gov (United States)

    Fu, Mingxuan; Imai, Takashi; Han, Tian-Heng; Lee, Young S

    2015-11-06

    The kagome Heisenberg antiferromagnet is a leading candidate in the search for a spin system with a quantum spin-liquid ground state. The nature of its ground state remains a matter of active debate. We conducted oxygen-17 single-crystal nuclear magnetic resonance (NMR) measurements of the spin-1/2 kagome lattice in herbertsmithite [ZnCu3(OH)6Cl2], which is known to exhibit a spinon continuum in the spin excitation spectrum. We demonstrated that the intrinsic local spin susceptibility χ(kagome), deduced from the oxygen-17 NMR frequency shift, asymptotes to zero below temperatures of 0.03J, where J ~ 200 kelvin is the copper-copper superexchange interaction. Combined with the magnetic field dependence of χ(kagome) that we observed at low temperatures, these results imply that the kagome Heisenberg antiferromagnet has a spin-liquid ground state with a finite gap.

  5. Long-range order for the spin-1 Heisenberg model with a small antiferromagnetic interaction

    Energy Technology Data Exchange (ETDEWEB)

    Lees, Benjamin, E-mail: b.lees@warwick.ac.uk [Department of Mathematics, University of Warwick, Coventry CV4 7AL (United Kingdom)

    2014-09-15

    We look at the general SU(2) invariant spin-1 Heisenberg model. This family includes the well-known Heisenberg ferromagnet and antiferromagnet as well as the interesting nematic (biquadratic) and the largely mysterious staggered-nematic interaction. Long range order is proved using the method of reflection positivity and infrared bounds on a purely nematic interaction. This is achieved through the use of a type of matrix representation of the interaction making clear several identities that would not otherwise be noticed. Using the reflection positivity of the antiferromagnetic interaction one can then show that the result is maintained if we also include an antiferromagnetic interaction that is sufficiently small.

  6. Frustration in a transverse Ising nanoisland with an antiferromagnetic spin configuration

    Energy Technology Data Exchange (ETDEWEB)

    Kaneyoshi, T., E-mail: kaneyosi@is.nagoya-u.ac.Jp

    2015-09-01

    The phase diagrams, saturation magnetizations and temperature dependences of magnetizations in a transverse Ising nanoisland with an antiferromagnetic spin configuration are studied by the uses of the effective-field theory with correlations (EFT) and the mean-field approximation (MFA), in order to clarify whether the MFA can be successfully applied to the theoretical discussions of naonoislands. From these investigations, we have found a lot of unexpected characteristic phenomena in these properties, when the value of an interlayer coupling takes a large value. We have also found that the applications of the MFA to the magnetic properties are extremely restricted for nanoislands, when the value of an interlayer coupling takes a large value, in contrast to a number of bulk studies.

  7. Boundary-induced spin-density waves in linear Heisenberg antiferromagnetic spin chains with S ≥1

    Science.gov (United States)

    Dey, Dayasindhu; Kumar, Manoranjan; Soos, Zoltán G.

    2016-10-01

    Linear Heisenberg antiferromagnets (HAFs) are chains of spin-S sites with isotropic exchange J between neighbors. Open and periodic boundary conditions return the same ground-state energy per site in the thermodynamic limit, but not the same spin SG when S ≥1 . The ground state of open chains of N spins has SG=0 or S , respectively, for even or odd N . Density-matrix renormalization-group calculations with different algorithms for even and odd N are presented up to N =500 for the energy and spin densities ρ (r ,N ) of edge states in HAFs with S =1 , 3/2, and 2. The edge states are boundary-induced spin density waves (BI-SDWs) with ρ (r ,N ) ∝(-1) r -1 for r =1 ,2 ,...,N . The SDWs are in phase when N is odd, are out of phase when N is even, and have finite excitation energy Γ (N ) that decreases exponentially with N for integer S and faster than 1 /N for half integer S . The spin densities and excitation energy are quantitatively modeled for integer S chains longer than 5 ξ spins by two parameters, the correlation length ξ and the SDW amplitude, with ξ =6.048 for S =1 and 49.0 for S =2 . The BI-SDWs of S =3 /2 chains are not localized and are qualitatively different for even and odd N . Exchange between the ends for odd N is mediated by a delocalized effective spin in the middle that increases |Γ (N )| and weakens the size dependence. The nonlinear sigma model (NL σ M ) has been applied to the HAFs, primarily to S =1 with even N , to discuss spin densities and exchange between localized states at the ends as Γ (N ) ∝(-1) Nexp(-N /ξ ) . S =1 chains with odd N are fully consistent with the NL σ M ; S =2 chains have two gaps Γ (N ) with the same ξ as predicted whose ratio is 3.45 rather than 3; the NL σ M is more approximate for S =3 /2 chains with even N and is modified for exchange between ends for odd N .

  8. Inducing spin-dependent tunneling to probe magnetic correlations in optical lattices

    DEFF Research Database (Denmark)

    Pedersen, Kim-Georg; Andersen, Brian; Syljuåsen, Olav;

    2012-01-01

    We suggest a simple experimental method for probing antiferromagnetic spin correlations of two-component Fermi gases in optical lattices. The method relies on a spin selective Raman transition to excite atoms of one spin species to their first excited vibrational mode where the tunneling is large...

  9. Intrinsic life-time and external manipulation of Néel states in antiferromagnetic adatom spins on semiconductor surfaces

    Science.gov (United States)

    Li, Jun; Liu, Bang-Gui

    2015-06-01

    It has been proposed that antiferromagnetic Fe adatom spins on semiconductor Cu-N surfaces can be used to store information (Loth et al 2012 Science 335 196). Here, we investigate spin dynamics of such antiferromagnetic systems through Monte Carlo simulations. We find out the temperature and size laws of switching rates of Néel states and show that the Néel states can become stable enough for the information storage when the number of spins reaches one or two dozens of the Fe spins. We also explore promising methods for manipulating the Néel states. These could help realize information storage with such antiferromagnetic spin systems.

  10. Quark spin-orbit correlations

    CERN Document Server

    Lorcé, Cédric

    2014-01-01

    The proton spin puzzle issue focused the attention on the parton spin and orbital angular momentum contributions to the proton spin. However, a complete characterization of the proton spin structure requires also the knowledge of the parton spin-orbit correlation. We showed that this quantity can be expressed in terms of moments of measurable parton distributions. Using the available phenomenological information about the valence quarks, we concluded that this correlation is negative, meaning that the valence quark spin and kinetic orbital angular momentum are, in average, opposite. The quark spin-orbit correlation can also be expressed more intuitively in terms of relativistic phase-space distributions, which can be seen as the mother distributions of the standard generalized and transverse-momentum dependent parton distributions. We present here for the first time some examples of the general multipole decomposition of these phase-space distributions.

  11. Giant electrothermal conductivity and spin-phonon coupling in an antiferromagnetic oxide.

    Science.gov (United States)

    Chiorescu, C; Neumeier, J J; Cohn, J L

    2008-12-19

    The application of weak electric fields ( less, similar 100 V/cm) is found to dramatically enhance the lattice thermal conductivity of the antiferromagnetic insulator CaMnO3 over a broad range of temperature about the Néel ordering point (125 K). The effect is coincident with field-induced detrapping of bound electrons, suggesting that phonon scattering associated with short- and long-ranged antiferromagnetic order is suppressed in the presence of the mobilized charge. This interplay between bound charge and spin-phonon coupling might allow for the reversible control of spin fluctuations using weak external fields.

  12. Bond-Dilution Effects on Two-Dimensional Spin-Gapped Heisenberg Antiferromagnets

    OpenAIRE

    Yasuda, Chitoshi; Todo, Synge; Matsumoto, Munehisa; Takayama, Hajime

    2001-01-01

    Bond-dilution effects on spin-1/2 spin-gapped Heisenberg antiferromagnets of coupled alternating chains on a square lattice are investigated by means of the quantum Monte Carlo method. It is found that, in contrast with the site-diluted system having an infinitesimal critical concentration, the bond-diluted system has a finite critical concentration of diluted bonds, $x_{c}$, above which the system is in an antiferromagnetic (AF) long-range ordered phase. In the disordered phase below $x_{c}$...

  13. Vectorial mapping of noncollinear antiferromagnetic structure of semiconducting FeSe surface with spin-polarized scanning tunneling microscopy

    Energy Technology Data Exchange (ETDEWEB)

    Zhang, K. F.; Yang, Fang; Song, Y. R. [Key Laboratory of Artificial Structures and Quantum Control (Ministry of Education), Department of Physics and Astronomy, Shanghai Jiao Tong University, Shanghai 200240 (China); Zhang, Xiaole [Institute of Natural Sciences, Shanghai Jiao Tong University, Shanghai 200240 (China); The State Key Laboratory of Advanced Optical Communication Systems and Networks, Department of Physics and Astronomy, Shanghai Jiao Tong University, Shanghai 200240 (China); Chen, Xianfeng [The State Key Laboratory of Advanced Optical Communication Systems and Networks, Department of Physics and Astronomy, Shanghai Jiao Tong University, Shanghai 200240 (China); Liu, Canhua; Qian, Dong; Gao, C. L., E-mail: clgao@sjtu.edu.cn; Jia, Jin-Feng [Key Laboratory of Artificial Structures and Quantum Control (Ministry of Education), Department of Physics and Astronomy, Shanghai Jiao Tong University, Shanghai 200240 (China); Collaborative Innovation Center of Advanced Microstructures, Nanjing (China); Luo, Weidong, E-mail: wdluo@sjtu.edu.cn [Key Laboratory of Artificial Structures and Quantum Control (Ministry of Education), Department of Physics and Astronomy, Shanghai Jiao Tong University, Shanghai 200240 (China); Institute of Natural Sciences, Shanghai Jiao Tong University, Shanghai 200240 (China); Collaborative Innovation Center of Advanced Microstructures, Nanjing (China)

    2016-02-08

    Antiferromagnetic semiconductors gain increasing interest due to their possible application in spintronics. Using spin polarized scanning tunneling microscopy operating in a vector field, we mapped the noncollinear antiferromagnetic spin structure of a semiconducting hexagonal FeSe surface on the atomic scale. The surface possesses an in-plane compensated Néel structure which is further confirmed by first-principles calculations.

  14. Thermoinduced magnetization and uncompensated spins in antiferromagnetic nanoparticles

    DEFF Research Database (Denmark)

    Madsen, Daniel Esmarch; Mørup, Steen

    2006-01-01

    We have investigated the combined effect of an uncompensated moment and the thermoinduced magnetization on the initial susceptibility of nanoparticles of antiferromagnetic materials. We find that for nanoparticles with small values of the anisotropy and exchange fields, the thermoinduced...... magnetization may be predominant at finite temperatures. In other cases the uncompensated moment may be predominant....

  15. Spin-orbit torques in locally and globally noncentrosymmetric crystals: Antiferromagnets and ferromagnets

    Science.gov (United States)

    Železný, J.; Gao, H.; Manchon, Aurélien; Freimuth, Frank; Mokrousov, Yuriy; Zemen, J.; Mašek, J.; Sinova, Jairo; Jungwirth, T.

    2017-01-01

    One of the main obstacles that prevents practical applications of antiferromagnets is the difficulty of manipulating the magnetic order parameter. Recently, following the theoretical prediction [J. Železný et al., Phys. Rev. Lett. 113, 157201 (2014)], 10.1103/PhysRevLett.113.157201, the electrical switching of magnetic moments in an antiferromagnet was demonstrated [P. Wadley et al., Science 351, 587 (2016)], 10.1126/science.aab1031. The switching is due to the so-called spin-orbit torque, which has been extensively studied in ferromagnets. In this phenomena a nonequilibrium spin-polarization exchange coupled to the ordered local moments is induced by current, hence exerting a torque on the order parameter. Here we give a general systematic analysis of the symmetry of the spin-orbit torque in locally and globally noncentrosymmetric crystals. We study when the symmetry allows for a nonzero torque, when is the torque effective, and its dependence on the applied current direction and orientation of magnetic moments. For comparison, we consider both antiferromagnetic and ferromagnetic orders. In two representative model crystals we perform microscopic calculations of the spin-orbit torque to illustrate its symmetry properties and to highlight conditions under which the spin-orbit torque can be efficient for manipulating antiferromagnetic moments.

  16. Spin-orbit torques in locally and globally noncentrosymmetric crystals: Antiferromagnets and ferromagnets

    KAUST Repository

    Železný, J.

    2017-01-10

    One of the main obstacles that prevents practical applications of antiferromagnets is the difficulty of manipulating the magnetic order parameter. Recently, following the theoretical prediction [J. Železný, Phys. Rev. Lett. 113, 157201 (2014)]PRLTAO0031-900710.1103/PhysRevLett.113.157201, the electrical switching of magnetic moments in an antiferromagnet was demonstrated [P. Wadley, Science 351, 587 (2016)]SCIEAS0036-807510.1126/science.aab1031. The switching is due to the so-called spin-orbit torque, which has been extensively studied in ferromagnets. In this phenomena a nonequilibrium spin-polarization exchange coupled to the ordered local moments is induced by current, hence exerting a torque on the order parameter. Here we give a general systematic analysis of the symmetry of the spin-orbit torque in locally and globally noncentrosymmetric crystals. We study when the symmetry allows for a nonzero torque, when is the torque effective, and its dependence on the applied current direction and orientation of magnetic moments. For comparison, we consider both antiferromagnetic and ferromagnetic orders. In two representative model crystals we perform microscopic calculations of the spin-orbit torque to illustrate its symmetry properties and to highlight conditions under which the spin-orbit torque can be efficient for manipulating antiferromagnetic moments.

  17. Ferromagnetic–ferromagnetic–antiferromagnetic–antiferromagnetic correlation and magnetization plateau in spin-1/2 J{sub 1}–J{sub 1}–J{sub 2}–J{sub 2} tetrameric chains

    Energy Technology Data Exchange (ETDEWEB)

    Deng, Xiao-Yan [Graduate School, Tianjin Polytechnic University, Tianjin 300387 (China); Dou, Jun-Ya [Department of Physics, Tianjin Polytechnic University, Tianjin 300387 (China); Liu, Guang-Hua, E-mail: liuguanghua@tjpu.edu.cn [Department of Physics, Tianjin Polytechnic University, Tianjin 300387 (China)

    2015-10-15

    The magnetization process of a spin-1/2 J{sub 1}–J{sub 1}–J{sub 2}–J{sub 2} tetrameric Heisenberg chain is investigated by the infinite time-evolving block decimation (iTEBD) method. A magnetization phase diagram including three different phases, i.e., a fully polarized (FP) phase, a 1/2 plateau phase, and a spin-fluid (SF) phase, is obtained. All the quantum phase transitions (QPTs) are determined to belong to the second-order category, and the central charge in the critical SF phase equals 1. In addition, a 1/2 plateau phase also exists in the classical J{sub 1}–J{sub 1}–J{sub 2}–J{sub 2} tetrameric Ising chain. The F–F–AF–AF (or AF–AF–F–F) type longitudinal correlation is found to be important and necessary for the appearance of the 1/2 plateau state in both quantum and classical cases. - Highlights: • 1/2 magnetization plateau can be realized in both quantum and classical cases. • 1/2 plateau is characterized by constant magnetization, entanglement and correlation. • Central charge of the spin-fluid phase is determined to be 1. • F–F–AF–AF correlation is important for the appearance of the 1/2 plateau.

  18. Effect of Quantum Fluctuation on Two-Dimensional Spatially Anisotropic Heisenberg Antiferromagnet with Integer Spin

    Institute of Scientific and Technical Information of China (English)

    JI An-Chun; TIAN Guang-Shan

    2006-01-01

    In the present paper, we calculate the Gaussian correction to the critical value Jc⊥ caused by quantum spin fluctuation in a two-dimensional spatially anisotropic Heisenberg antiferromagnet with integer spin S. Previously, someauthors computed this quantity by the mean-field theory based on the Schwinger boson representation of spin operators.However, for S = 1, their result is much less than the one derived by numerical calculations. By taking the effect ofquantum spin fluctuation into consideration, we are able to produce a greatly improved result.

  19. Low Energy Properties of the Random Spin-1/2 Ferromagnetic-Antiferromagnetic Heisenberg Chain

    OpenAIRE

    Hida, Kazuo

    1996-01-01

    The low energy properties of the spin-1/2 random Heisenberg chain with ferromagnetic and antiferromagnetic interactions are studied by means of the density matrix renormalization group (DMRG) and real space renormalization group (RSRG) method for finite chains. The results of the two methods are consistent with each other. The deviation of the gap distribution from that of the random singlet phase and the formation of the large-spin state is observed even for relatively small systems. For a s...

  20. The magnetic properties of the spin-1 Heisenberg antiferromagnetic chain with single-ion anisotropy

    Energy Technology Data Exchange (ETDEWEB)

    Hu, Gangsan; Zhu, Rengui, E-mail: rgzhu@mail.ahnu.edu.cn

    2015-02-15

    The magnetic properties of the spin-1 Heisenberg antiferromagnetic chain with exchange anisotropy and single-ion anisotropy are studied by the double-time Green's function method. The determinative equations for the critical temperature, the magnetization, and the zero-field susceptibility are derived analytically. The effects of the anisotropies on the magnetic properties are presented.

  1. Room temperature spin-polarizations of Mn-based antiferromagnetic nanoelectrodes

    Energy Technology Data Exchange (ETDEWEB)

    Yamada, Toyo Kazu, E-mail: toyoyamada@faculty.chiba-u.jp [Graduate School of Advanced Integration Science, Chiba University, 1-33, Yayoi-cho, Inage-ku, Chiba-shi 263-8522, Chiba (Japan); Vazquez de Parga, Amadeo L. [Instituto Madrileño de Estudios Avanzados en Nanociencia IMDEA-Nanociencia and Dep. Fisica de la Materia Condensada, Universidad Autónoma de Madrid, Cantoblanco, 28049 Madrid (Spain)

    2014-11-03

    Antiferromagnets produce no stray field, and therefore, a tip electrode made of antiferromagnetic material has been considered to be the most suitable choice to measure such as magnetoresistance (MR) through single isolated magnetic nanoparticles, molecules, and ultrathin films. Spin polarizations (P) of antiferromagnetic 3-nm, 6-nm, and annealed 3-nm Mn films grown on W tips with a bcc(110) apex as well as bulk-NiMn tips were obtained at 300 K by measuring MR in ultrahigh vacuum by means of spin-polarized scanning tunneling microscopy using a layerwise antiferromagnetically stacking bct-Mn(001) film electrode. The Mn-coated tips with coverages of 3 and 6 nm exhibited P values of 1 ± 1% and 3 ± 2%, respectively, which tips likely contain α- or strained Mn. With a thermal assist, the crystalline quality and the magnetic stability of the film could increase. The annealed tip exhibited P = 9 ± 2%. The bulk-NiMn tips exhibit spin polarizations of 0 or 6 ± 2% probably depending on the chemical species (Mn or Ni) present at the apex of the tip. Fe-coated W tips were used to estimate the bct-Mn(001) film spin polarization.

  2. STUDIES OF FCC HEISENBERG ANTIFERROMAGNETS BY MONTE CARLO SIMULATION ON LARGE SPIN ARRAYS

    OpenAIRE

    Minor, W.; Giebultowicz, T.

    1988-01-01

    We report Monte Carlo studies of fcc Heisenberg antiferromagnets carried out on arrays with 108,000 spins. A lattice with only JNN ≠ 0 was found to exhibit a Type I AF order despite the disordered nature of its ground state. Contrary to previous reports, our data indicate in this case a first order phase transition.

  3. Barlowite: A Spin-1/2 Antiferromagnet with a Geometrically Perfect Kagome Motif.

    Science.gov (United States)

    Han, Tian-Heng; Singleton, John; Schlueter, John A

    2014-11-28

    We present thermodynamic studies of a new spin-1/2 antiferromagnet containing undistorted kagome lattices-barlowite Cu_{4}(OH)_{6}FBr. Magnetic susceptibility gives θ_{CW}=-136  K, while long-range order does not happen until T_{N}=15  K with a weak ferromagnetic moment μkagome lattice makes charge doping promising.

  4. Electric Control of Dirac Quasiparticles by Spin-Orbit Torque in an Antiferromagnet

    Science.gov (United States)

    Šmejkal, L.; Železný, J.; Sinova, J.; Jungwirth, T.

    2017-03-01

    Spin orbitronics and Dirac quasiparticles are two fields of condensed matter physics initiated independently about a decade ago. Here we predict that Dirac quasiparticles can be controlled by the spin-orbit torque reorientation of the Néel vector in an antiferromagnet. Using CuMnAs as an example, we formulate symmetry criteria allowing for the coexistence of topological Dirac quasiparticles and Néel spin-orbit torques. We identify the nonsymmorphic crystal symmetry protection of Dirac band crossings whose on and off switching is mediated by the Néel vector reorientation. We predict that this concept verified by minimal model and density functional calculations in the CuMnAs semimetal antiferromagnet can lead to a topological metal-insulator transition driven by the Néel vector and to the topological anisotropic magnetoresistance.

  5. Spin-1/2 Heisenberg Antiferromagnet on the Spatially Anisotropic Kagome Lattice

    Science.gov (United States)

    Schnyder, Andreas; Starykh, Oleg; Balents, Leon

    2008-03-01

    We study the quasi-one-dimensional limit of the Spin-1/2 quantum antiferromagnet on the Kagome lattice, a model Hamiltonian that might be of relevance for the mineral volborthite [1,2]. The lattice is divided into antiferromagnetic spin-chains (exchange J) that are weakly coupled via intermediate ``dangling'' spins (exchange J'). Using bosonization, renormalization group methods, and current algebra techniques we determine the ground state as a function of J'/J. The case of a strictly one-dimensional Kagome strip is also discussed. [1] Z. Hiroi, M. Hanawa, N. Kobayashi, M. Nohara, Hidenori Takagi, Y. Kato, and M. Takigawa, J. Phys. Soc. Japan 70, 3377 (2001). [2] F. Bert, D. Bono, P. Mendels, F. Ladieu, F. Duc, J.-C. Trumbe, and P. Millet, Phys. Rev. Lett. 95, 087203 (2005).

  6. Spin Correlation in Binary Systems

    CERN Document Server

    Farbiash, N; Farbiash, Netzach; Steinitz, Raphael

    2004-01-01

    We examine the correlation of projected rotational velocities in binary systems. It is an extension of previous work (Steinitz and Pyper, 1970; Levato, 1974). An enlarged data basis and new tests enable us to conclude that there is indeed correlation between the projected rotational velocities of components of binaries. In fact we suggest that spins are already correlated.

  7. Spin transport of the frustrated quasi-two-dimensional XY-like antiferromagnet

    Science.gov (United States)

    Lima, L. S.

    2017-01-01

    We use the Self Consistent Harmonic Approximation together with the Kubo formalism of the Linear Response Theory to study the spin transport in the two-dimensional frustrated Heisenberg antiferromagnet in a square lattice with easy-plane ion single anisotropy. The regular part of the spin conductivity σreg(ω) is determined for several values of the critical ion single parameter Dc, that separates the low D region from the large D quantum paramagnetic phase. We have obtained an abrupt change in the spin conductivity in the discontinuity points of the graphic Dc vs. η, where the system presents a quantum phase transition.

  8. Correlation-Mediated Processes for Electron-Induced Switching between Néel States of Fe Antiferromagnetic Chains

    Science.gov (United States)

    Gauyacq, Jean-Pierre; Yaro, Simeón Moisés; Cartoixà, Xavier; Lorente, Nicolás

    2013-02-01

    The controlled switching between two quasistable Néel states in adsorbed antiferromagnetic Fe chains has recently been achieved by Loth et al. [Science 335, 196 (2012)SCIEAS0036-8075] using tunneling electrons from an STM tip. In order to rationalize their data, we evaluate the rate of tunneling electron-induced switching between the Néel states. Good agreement is found with the experiment, permitting us to identify three switching mechanisms: (i) low STM voltage direct electron-induced transitions, (ii) intermediate STM voltage switching via spin-wave-like excitation, and (iii) high STM voltage transitions mediated by domain-wall formation. Spin correlations in the antiferromagnetic chains are the switching driving force, leading to a marked chain-size dependence.

  9. Dynamic selective switching in antiferromagnetically-coupled bilayers close to the spin reorientation transition

    Energy Technology Data Exchange (ETDEWEB)

    Fernández-Pacheco, A., E-mail: af457@cam.ac.uk; Mansell, R.; Petit, D.; Lee, J. H.; Cowburn, R. P. [Cavendish Laboratory, University of Cambridge, J. J. Thomson Avenue, Cambridge CB3 0HE (United Kingdom); Ummelen, F. C.; Swagten, H. J. M. [Department of Applied Physics, Center for NanoMaterials, Eindhoven University of Technology, P.O. Box 513, 5600 MB Eindhoven (Netherlands)

    2014-09-01

    We have designed a bilayer synthetic antiferromagnet where the order of layer reversal can be selected by varying the sweep rate of the applied magnetic field. The system is formed by two ultra-thin ferromagnetic layers with different proximities to the spin reorientation transition, coupled antiferromagnetically using Ruderman-Kittel-Kasuya-Yosida interactions. The different dynamic magnetic reversal behavior of both layers produces a crossover in their switching fields for field rates in the kOe/s range. This effect is due to the different effective anisotropy of both layers, added to an appropriate asymmetric antiferromagnetic coupling between them. Field-rate controlled selective switching of perpendicular magnetic anisotropy layers as shown here can be exploited in sensing and memory applications.

  10. Superconductivity, antiferromagnetism, and neutron scattering

    Energy Technology Data Exchange (ETDEWEB)

    Tranquada, John M., E-mail: jtran@bnl.gov; Xu, Guangyong; Zaliznyak, Igor A.

    2014-01-15

    High-temperature superconductivity in both the copper-oxide and the iron–pnictide/chalcogenide systems occurs in close proximity to antiferromagnetically ordered states. Neutron scattering has been an essential technique for characterizing the spin correlations in the antiferromagnetic phases and for demonstrating how the spin fluctuations persist in the superconductors. While the nature of the spin correlations in the superconductors remains controversial, the neutron scattering measurements of magnetic excitations over broad ranges of energy and momentum transfers provide important constraints on the theoretical options. We present an overview of the neutron scattering work on high-temperature superconductors and discuss some of the outstanding issues. - Highlights: • High-temperature superconductivity is closely associated with antiferromagnetism. • Antiferromagnetic spin fluctuations coexist with the superconductivity. • Neutron scattering is essential for characterising the full spectrum of spin excitations.

  11. Competing antiferromagnetic and spin-glass phases in a hollandite structure

    Science.gov (United States)

    Crespo, Y.; Andreanov, A.; Seriani, N.

    2013-07-01

    We introduce a simple lattice model with Ising spins as a zeroth-order approximation of the hollandite-type magnetic compounds. We argue that geometrical frustration of the lattice in combination with nearest-neighbor antiferromagnetic (AFM) interactions are responsible for the appearance of a spin-glass phase in presence of disorder. We investigate this system numerically using parallel tempering. The model reproduces magnetic transitions present in some oxides with hollandite structure and displays a rich phenomenology: in the absence of disorder we have identified five different ground states, depending on the relative strength and sign of the interactions: one ferromagnetically ordered, three antiferromagnetically ordered, and one disordered, macroscopically degenerate ground state. Remarkably, for the sets of AFM couplings having an AFM ground state in the clean system, there exists a critical value of the disorder above which the ground state becomes a spin glass while maintaining all the couplings antiferromagnetically. This model presents this kind of transition with nearest-neighbor frustrated AFM interactions. We argue that this model is useful for understanding the relation between AFM coupling, disorder, and appearance of spin-glass phases.

  12. Itinerant spin dynamics in iron-based superconductors and cerium-based heavy-fermion antiferromagnets

    Energy Technology Data Exchange (ETDEWEB)

    Friemel, Gerd

    2014-05-26

    This thesis contains a comprehensive study of the spin excitations by inelastic neutron scattering (INS) in two different correlated electron systems: the alkali-metal iron selenide superconductors (FeSe122) A{sub x}Fe{sub 2-y}Se{sub 2} (A=K, Rb, Cs) and the heavy-fermion antiferromagnet CeB6. Both systems exhibit intense modes in their spin-fluctuation spectrum below their respective transition temperatures that can be derived from the spin dynamics of the itinerant quasiparticles. However, the implications of these observations, presented here, are different for each particular compound. The A{sub x}Fe{sub 2-y}Se{sub 2} superconductors, with a uniform T{sub c} of 32 K, belong to a qualitative new family of superconductors. They possess a distinctly different Fermi surface compared to the iron-arsenide-based analogues XFe{sub 2}As{sub 2} (X=Ca, Sr, Ba). Instead of the central hole pockets at Γ and the electron pockets at X((1)/(2) 0), which are nested by the Q{sub AFM} = ((1)/(2) 0) vector, there exist only large electron pockets at the X point. Therefore, the magnetic instability along Q{sub AFM} that presumably provides the pairing glue for the superconductivity in the shape of spin fluctuations is absent in the FeSe122. The search for spin fluctuations by INS was motivated by a theoretical analysis that predicted their presence at an incommensurate wave vector near Q = (0.5 δ), δ = 0.3125 which results from a quasinesting by Q between the flat parts of the electron pockets. Two samples, namely Rb{sub 0.8}Fe{sub 1.6}Se{sub 2} and K{sub 0.77}Fe{sub 1.85}Se{sub 2}, were prepared and both showed a sizable anisotropic magnetic response at Q{sub sf} = ((1)/(2) (1)/(4)) in the normal state. Furthermore, upon entering the superconducting (SC) state a strong excitation appears at ℎω{sub res} = 14 meV in the spectrum at Q{sub sf}, which is referred to as magnetic resonant mode. This mode is interpreted as a bound spin-1 exciton below the SC charge gap. Its presence

  13. Antiferromagnetic order and spin glass behavior in Dy{sub 2}CuIn{sub 3}

    Energy Technology Data Exchange (ETDEWEB)

    Siouris, I.M., E-mail: jsiou@pme.duth.gr [Democritus University of Thrace (DUTH), Production and Management Engineering Department, Materials Laboratory, 67100 Xanthi (Greece); Kremer, R.K. [Max-Planck-Institut fuer Festkoerperforschung, Heisenbergstrasse 1, D-70569 Stuttgart (Germany); Hoelzel, M. [Technische Universitaet Muenchen, Forschungsneutronenquelle Heinz Maier-Leibnitz (FRM II), 85748 Garching (Germany)

    2011-11-15

    The magnetic properties of the intermetallic compound Dy{sub 2}CuIn{sub 3} have been investigated. Ac and dc-susceptibility measurements indicate an onset of antiferromagnetic ordering at T{sub N}=19.5 K and an additional frequency dependent transition at T{sub ds}{approx}9 K. Neutron diffraction studies confirm the ordered transition at 19.5{+-}1 K. The magnetic unit cell can be described by the propagation vector k=(0.25,0.25,0) with the magnetic moment {mu}=2.63(4){mu}{sub B}/Dy{sup 3+} parallel to the c-axis. Nevertheless, neutron diffraction reveals no additional magnetic phase transition around or below 9 K, which suggests that, at lower temperatures, a spin glass state may be formed in coexistence with the antiferromagnetic mode as a result of frustration and the antagonism between ferromagnetic and antiferromagnetic exchange interactions. - Highlights: > Dy{sub 2}CuIn{sub 3} is characterized by the dominance of antiferromagnetic (AF) interactions. > Geometric frustration and crystal field effects prevent the formation of the full magnetic moment on the Dy ions. > Two magnetic regimes are recognized: an AF state and a mixed AF-glassy state. > The antiferromagnetic structure of the compound has been determined.

  14. Spin-polarized valley Hall effect in ultrathin silicon nanomembrane via interlayer antiferromagnetic coupling

    Science.gov (United States)

    Sun, Jia-Tao; Wang, Zhengfei; Meng, S.; Du, Shixuan; Liu, F.; Gao, H.-J.

    2016-09-01

    Fundamental understanding of two-dimensional materials has spurred a surge in the search for topological quantum phase associated with the valley degree of freedom (VDOF). We discuss a spin-polarized version to the VDOF in which spin degeneracy is broken by the antiferromagnetic exchange coupling (LAFM) between opposite layers of the quasi-two-dimensional silicon nanomembrane (SiNM). Based on first principles calculations, we found that the LAFM state in SiNM can lead to metal-insulator transition (MIT). The broken degeneracy of spin degree of freedom in this insulating state of ultrathin SiNM may differ for different valleys, so that the SiNM can be exploited to produce the spatially separated spin and valley currents. We propose that the tunable spin-polarized valley photocurrents can be generated in an experimentally feasible ellipsometry setup. Our work shows promise for the development of spintronic and valleytronic devices compatible with current silicon industry.

  15. Antiferromagnetic spintronics.

    Science.gov (United States)

    Jungwirth, T; Marti, X; Wadley, P; Wunderlich, J

    2016-03-01

    Antiferromagnetic materials are internally magnetic, but the direction of their ordered microscopic moments alternates between individual atomic sites. The resulting zero net magnetic moment makes magnetism in antiferromagnets externally invisible. This implies that information stored in antiferromagnetic moments would be invisible to common magnetic probes, insensitive to disturbing magnetic fields, and the antiferromagnetic element would not magnetically affect its neighbours, regardless of how densely the elements are arranged in the device. The intrinsic high frequencies of antiferromagnetic dynamics represent another property that makes antiferromagnets distinct from ferromagnets. Among the outstanding questions is how to manipulate and detect the magnetic state of an antiferromagnet efficiently. In this Review we focus on recent works that have addressed this question. The field of antiferromagnetic spintronics can also be viewed from the general perspectives of spin transport, magnetic textures and dynamics, and materials research. We briefly mention this broader context, together with an outlook of future research and applications of antiferromagnetic spintronics.

  16. Spin squeezing and quantum correlations

    Indian Academy of Sciences (India)

    K S Mallesh; Swarnamala Sirsi; Mahmoud A A Sbaih; P N Deepak; G Ramachandran

    2002-08-01

    We discuss the notion of spin squeezing considering two mutually exclusive classes of spin- states, namely, oriented and non-oriented states. Our analysis shows that the oriented states are not squeezed while non-oriented states exhibit squeezing. We also present a new scheme for construction of spin- states using 2 spinors oriented along different axes. Taking the case of = 1, we show that the `non-oriented’ nature and hence squeezing arise from the intrinsic quantum correlations that exist among the spinors in the coupled state.

  17. Pairing Correlations at High Spins

    Science.gov (United States)

    Ma, Hai-Liang; Dong, Bao-Guo; Zhang, Yan; Fan, Ping; Yuan, Da-Qing; Zhu, Shen-Yun; Zhang, Huan-Qiao; Petrache, C. M.; Ragnarsson, I.; Carlsson, B. G.

    The pairing correcting energies at high spins in 161Lu and 138Nd are studied by comparing the results of the cranked-Nilsson-Strutinsky (CNS) and cranked-Nilsson-Strutinsky-Bogoliubov (CNSB) models. It is concluded that the Coriolis effect rather than the rotational alignment effect plays a major role in the reduction of the pairing correlations in the high spin region. Then we proposed an average pairing correction method which not only better reproduces the experimental data comparing with the CNS model but also enables a clean-cut tracing of the configurations thus the full-spin-range discussion on the various rotating bands.

  18. The antiferromagnetic cross-coupled spin ladder: Quantum fidelity and tensor networks approach

    Science.gov (United States)

    Chen, Xi-Hao; Cho, Sam Young; Zhou, Huan-Qiang; Batchelor, Murray T.

    2016-05-01

    We investigate the phase diagram of the cross-coupled Heisenberg spin ladder with antiferromagnetic couplings. For this model, the results for the existence of the columnar dimer phase, which was predicted on the basis of weak coupling field theory renormalization group arguments, have been conflicting. The numerical work on this model has been based on various approaches, including exact diagonalization, series expansions and density-matrix renormalization group calculations. Using the recently-developed tensor network states and groundstate fidelity approach for quantum spin ladders, we find no evidence for the existence of the columnar dimer phase. We also provide an argument based on the symmetry of the Hamiltonian, which suggests that the phase diagram for antiferromagnetic couplings consists of a single line separating the rung-singlet and the Haldane phases.

  19. su(1,2) Algebraic Structure of XYZ Antiferromagnetic Model in Linear Spin-Wave Frame

    Institute of Scientific and Technical Information of China (English)

    GUAN Yong; JIN Shuo; LIN Bing-Sheng; XIE Bing-Hao; JING Si-Cong; YU Zhao-Xian; HOU Jing-Min

    2008-01-01

    The XYZ antiferromagnetic model in linear spin-wave frame is shown explicitly to have an su(1,2) aigebraic structure: the Hamiltonian can be written as a linear function of the su(1,2) algebra generators. Based on it, the energy eigenvalues are obtained by making use of the similar transformations, and the algebraic diagonalization method is investigated. Some numerical solutions are given, and the results indicate that only one group solution could be accepted in physics.

  20. Modified Spin Wave Thoery of the Bilayer Square Lattice Frustrated Quantum Heisenberg Antiferromagnet

    OpenAIRE

    Hida, Kazuo

    1995-01-01

    The ground state of the square lattice bilayer quantum antiferromagnet with nearest and next-nearest neighbour intralayer interaction is studied by means of the modified spin wave method. For weak interlayer coupling, the ground state is found to be always magnetically ordered while the quantum disordered phase appear for large enough interlayer coupling. The properties of the disordered phase vary according to the strength of the frustration. In the regime of weak frustration, the disordered...

  1. Susceptibility of the 2D spin-1 / 2 Heisenberg antiferromagnet with an impurity.

    Science.gov (United States)

    Höglund, Kaj H; Sandvik, Anders W

    2003-08-15

    We use a quantum Monte Carlo method (stochastic series expansion) to study the effects of a magnetic or nonmagnetic impurity on the magnetic susceptibility of the two-dimensional Heisenberg antiferromagnet. At low temperatures, we find a log-divergent contribution to the transverse susceptibility. We also introduce an effective few-spin model that can quantitatively capture the differences between magnetic and nonmagnetic impurities at high and intermediate temperatures.

  2. Enhancement of antiferromagnetic spin wave in the heavy-fermion superconductors

    Science.gov (United States)

    Koh, Shun-ichiro

    2000-06-01

    Recently, the inelastic neutron scattering experiments of UPd 2Al 3 showed that a sharp peak indicating a magnetic excitation appears below the superconducting phase transition temperature (M. Metoki et al., J. Phys. Soc. Japan 66 (1997) 2560, N. Bernhoeft et al., Phys. Rev. Lett. 81 (1998) 4244). Assuming this excitation to be an antiferromagnetic (AFM) spin wave, this paper deals with its enhancement by the superconductivity.

  3. Spin flop in one-dimensional Heisenberg antiferromagnet KCuF3

    Institute of Scientific and Technical Information of China (English)

    Shi Qing-Fan; Li Liang-Sheng; Wang Qi

    2004-01-01

    Following Yamada and Karo [J. Phys. Soc. Japan 63 (1994) 289], we have calculated the frequency-field diagram of antiferromagnetic resonance of KCuF3 using an eight-sublattice model and mean field approximation. A spin flop is found to take place from the [110]p to a direction perpendicular to [110]p in the c-plane at H≌ 42172A-m, which is in good agreement with the data obtained by measuring magnetic susceptibility.

  4. Spin flop in one-dimensional Heisenberg antiferromagnet KCuF3

    Science.gov (United States)

    Shi, Qing-Fan; Li, Liang-Sheng; Wang, Qi

    2004-04-01

    Following Yamada and Kato [J. Phys. Soc. Japan 63 (1994) 289], we have calculated the frequency-field diagram of antiferromagnetic resonance of KCuF3 using an eight-sublattice model and mean field approximation. A spin flop is found to take place from the [110]p to a direction perpendicular to [110]p in the c-plane at Hsimeq 42172A/m, which is in good agreement with the data obtained by measuring magnetic susceptibility.

  5. Spin-Lattice-Coupled Order in Heisenberg Antiferromagnets on the Pyrochlore Lattice.

    Science.gov (United States)

    Aoyama, Kazushi; Kawamura, Hikaru

    2016-06-24

    Effects of local lattice distortions on the spin ordering are investigated for the antiferromagnetic classical Heisenberg model on the pyrochlore lattice. It is found by Monte Carlo simulations that the spin-lattice coupling (SLC) originating from site phonons induces a first-order transition into two different types of collinear magnetic ordered states. The state realized at the stronger SLC is cubic symmetric characterized by the magnetic (1/2,1/2,1/2) Bragg peaks, while that at the weaker SLC is tetragonal symmetric characterized by the (1,1,0) ones, each accompanied by the commensurate local lattice distortions. Experimental implications to chromium spinels are discussed.

  6. Spin-Lattice-Coupled Order in Heisenberg Antiferromagnets on the Pyrochlore Lattice

    Science.gov (United States)

    Aoyama, Kazushi; Kawamura, Hikaru

    2016-06-01

    Effects of local lattice distortions on the spin ordering are investigated for the antiferromagnetic classical Heisenberg model on the pyrochlore lattice. It is found by Monte Carlo simulations that the spin-lattice coupling (SLC) originating from site phonons induces a first-order transition into two different types of collinear magnetic ordered states. The state realized at the stronger SLC is cubic symmetric characterized by the magnetic (1/2 ,1/2 ,1/2 ) Bragg peaks, while that at the weaker SLC is tetragonal symmetric characterized by the (1,1,0) ones, each accompanied by the commensurate local lattice distortions. Experimental implications to chromium spinels are discussed.

  7. Neutron spin-echo study of the critical dynamics of spin-5/2 antiferromagnets in two and three dimensions

    Science.gov (United States)

    Tseng, K. F.; Keller, T.; Walters, A. C.; Birgeneau, R. J.; Keimer, B.

    2016-07-01

    We report a neutron spin-echo study of the critical dynamics in the S =5/2 antiferromagnets MnF2 and Rb2MnF4 with three-dimensional (3D) and two-dimensional (2D) spin systems, respectively, in zero external field. Both compounds are Heisenberg antiferromagnets with a small uniaxial anisotropy resulting from dipolar spin-spin interactions, which leads to a crossover in the critical dynamics close to the Néel temperature, TN. By taking advantage of the μ eV energy resolution of the spin-echo spectrometer, we have determined the dynamical critical exponents z for both longitudinal and transverse fluctuations. In MnF2, both the characteristic temperature for crossover from 3D Heisenberg to 3D Ising behavior and the exponents z in both regimes are consistent with predictions from the dynamical scaling theory. The amplitude ratio of longitudinal and transverse fluctuations also agrees with predictions. In Rb2MnF4 , the critical dynamics crosses over from the expected 2D Heisenberg behavior for T ≫TN to a scaling regime with exponent z =1.387 (4 ) , which has not been predicted by theory and may indicate the influence of long-range dipolar interactions.

  8. Correlation-driven transport asymmetries through coupled spins in a tunnel junction

    Science.gov (United States)

    Muenks, Matthias; Jacobson, Peter; Ternes, Markus; Kern, Klaus

    2017-01-01

    Spin-spin correlations can be the driving force that favours certain ground states and are key in numerous models that describe the behaviour of strongly correlated materials. While the sum of collective correlations usually lead to a macroscopically measurable change in properties, a direct quantification of correlations in atomic scale systems is difficult. Here we determine the correlations between a strongly hybridized spin impurity on the tip of a scanning tunnelling microscope and its electron bath by varying the coupling to a second spin impurity weakly hybridized to the sample surface. Electronic transport through these coupled spins reveals an asymmetry in the differential conductance reminiscent of spin-polarized transport in a magnetic field. We show that at zero field, this asymmetry can be controlled by the coupling strength and is related to either ferromagnetic or antiferromagnetic spin-spin correlations in the tip.

  9. Antiferromagnetic nuclear spin helix and topological superconductivity in 13C nanotubes

    Science.gov (United States)

    Hsu, Chen-Hsuan; Stano, Peter; Klinovaja, Jelena; Loss, Daniel

    2015-12-01

    We investigate the Ruderman-Kittel-Kasuya-Yosida (RKKY) interaction arising from the hyperfine coupling between localized nuclear spins and conduction electrons in interacting 13C carbon nanotubes. Using the Luttinger liquid formalism, we show that the RKKY interaction is sublattice dependent, consistent with the spin susceptibility calculation in noninteracting carbon nanotubes, and it leads to an antiferromagnetic nuclear spin helix in finite-size systems. The transition temperature reaches up to tens of mK, due to a strong boost by a positive feedback through the Overhauser field from ordered nuclear spins. Similar to GaAs nanowires, the formation of the helical nuclear spin order gaps out half of the conduction electrons, and is therefore observable as a reduction of conductance by a factor of 2 in a transport experiment. The nuclear spin helix leads to a density wave combining spin and charge degrees of freedom in the electron subsystem, resulting in synthetic spin-orbit interaction, which induces nontrivial topological phases. As a result, topological superconductivity with Majorana fermion bound states can be realized in the system in the presence of proximity-induced superconductivity without the need of fine tuning the chemical potential. We present the phase diagram as a function of system parameters, including the pairing gaps, the gap due to the nuclear spin helix, and the Zeeman field perpendicular to the helical plane.

  10. Order-disorder quantum phase transition in the quasi-one-dimensional spin-1/2 collinear antiferromagnetic Heisenberg model.

    Science.gov (United States)

    Rufo, Sabrina; Mendonça, Griffith; Plascak, J A; de Sousa, J Ricardo

    2013-09-01

    The ground-state properties of the quasi-one-dimensional spin-1/2 antiferromagnetic Heisenberg model is investigated by using a variational method. Spins on chains along the x direction are antiferromagnetically coupled with exchange J>0, while spins between chains in the y direction are coupled either ferromagnetically (J' 0). The staggered and the colinear antiferromagnetic magnetizations are computed and their dependence on the anisotropy parameter λ=|J'|/J is analyzed. It is found that an infinitesimal interchain coupling parameter is sufficient to stabilize a long-range order with either a staggered magnetization m_{s} (J' > 0) or a colinear antiferromagnetic magnetization m_{caf} (J' < 0), both behaving as ≃λ¹/² for λ → 0.

  11. Antiferromagnetic Ising spin glass competing with BCS pairing interaction in a transverse field

    Science.gov (United States)

    Magalhães, S. G.; Zimmer, F. M.; Kipper, C. J.; Calegari, E. J.

    2006-07-01

    The competition among spin glass (SG), antiferromagnetism (AF) and local pairing superconductivity (PAIR) is studied in a two-sublattice fermionic Ising spin glass model with a local BCS pairing interaction in the presence of an applied magnetic transverse field Γ. In the present approach, spins in different sublattices interact with a Gaussian random coupling with an antiferromagnetic mean J0 and standard deviation J. The problem is formulated in the path integral formalism in which spin operators are represented by bilinear combinations of Grassmann variables. The saddle-point Grand Canonical potential is obtained within the static approximation and the replica symmetric ansatz. The results are analysed in phase diagrams in which the AF and the SG phases can occur for small g (g is the strength of the local superconductor coupling written in units of J), while the PAIR phase appears as unique solution for large g. However, there is a complex line transition separating the PAIR phase from the others. It is second order at high temperature that ends in a tricritical point. The quantum fluctuations affect deeply the transition lines and the tricritical point due to the presence of Γ.

  12. Thermal evolution of antiferromagnetic correlations and tetrahedral bond angles in superconducting FeTe1 -xSex

    Science.gov (United States)

    Xu, Zhijun; Schneeloch, J. A.; Wen, Jinsheng; Božin, E. S.; Granroth, G. E.; Winn, B. L.; Feygenson, M.; Birgeneau, R. J.; Gu, Genda; Zaliznyak, I. A.; Tranquada, J. M.; Xu, Guangyong

    2016-03-01

    It has recently been demonstrated that dynamical magnetic correlations measured by neutron scattering in iron chalcogenides can be described with models of short-range correlations characterized by particular choices of four-spin plaquettes, where the appropriate choice changes as the parent material is doped towards superconductivity. Here we apply such models to describe measured maps of magnetic scattering as a function of two-dimensional wave vectors obtained for optimally superconducting crystals of FeTe1 -xSex . We show that the characteristic antiferromagnetic wave vector evolves from that of the bicollinear structure found in underdoped chalcogenides (at high temperature) to that associated with the stripe structure of antiferromagnetic iron arsenides (at low temperature); these can both be described with the same local plaquette, but with different interplaquette correlations. While the magnitude of the low-energy magnetic spectral weight is substantial at all temperatures, it actually weakens somewhat at low temperature, where the charge carriers become more itinerant. The observed change in spin correlations is correlated with the dramatic drop in the electronic scattering rate and the growth of the bulk nematic response upon cooling. Finally, we also present powder neutron diffraction results for lattice parameters in FeTe1 -xSex indicating that the tetrahedral bond angle tends to increase towards the ideal value upon cooling, in agreement with the increased screening of the crystal field by more itinerant electrons and the correspondingly smaller splitting of the Fe 3 d orbitals.

  13. Spin wave dynamics in Heisenberg ferromagnetic/antiferromagnetic single-walled nanotubes

    Science.gov (United States)

    Mi, Bin-Zhou

    2016-09-01

    The spin wave dynamics, including the magnetization, spin wave dispersion relation, and energy level splitting, of Heisenberg ferromagnetic/antiferromagnetic single-walled nanotubes are systematically calculated by use of the double-time Green's function method within the random phase approximation. The role of temperature, diameter of the tube, and wave vector on spin wave energy spectrum and energy level splitting are carefully analyzed. There are two categories of spin wave modes, which are quantized and degenerate, and the total number of independent magnon branches is dependent on diameter of the tube, caused by the physical symmetry of nanotubes. Moreover, the number of flat spin wave modes increases with diameter of the tube rising. The spin wave energy and the energy level splitting decrease with temperature rising, and become zero as temperature reaches the critical point. At any temperature, the energy level splitting varies with wave vector, and for a larger wave vector it is smaller. When pb=π, the boundary of first Brillouin zone, spin wave energies are degenerate, and the energy level splittings are zero.

  14. Spin wave dynamics in Heisenberg ferromagnetic/antiferromagnetic single-walled nanotubes

    Energy Technology Data Exchange (ETDEWEB)

    Mi, Bin-Zhou, E-mail: mbzfjerry2008@126.com [Department of Basic Curriculum, North China Institute of Science and Technology, Beijing 101601 (China); Department of Physics, School of Mathematics and Physics, University of Science and Technology Beijing, Beijing 100083 (China)

    2016-09-15

    The spin wave dynamics, including the magnetization, spin wave dispersion relation, and energy level splitting, of Heisenberg ferromagnetic/antiferromagnetic single-walled nanotubes are systematically calculated by use of the double-time Green’s function method within the random phase approximation. The role of temperature, diameter of the tube, and wave vector on spin wave energy spectrum and energy level splitting are carefully analyzed. There are two categories of spin wave modes, which are quantized and degenerate, and the total number of independent magnon branches is dependent on diameter of the tube, caused by the physical symmetry of nanotubes. Moreover, the number of flat spin wave modes increases with diameter of the tube rising. The spin wave energy and the energy level splitting decrease with temperature rising, and become zero as temperature reaches the critical point. At any temperature, the energy level splitting varies with wave vector, and for a larger wave vector it is smaller. When pb=π, the boundary of first Brillouin zone, spin wave energies are degenerate, and the energy level splittings are zero.

  15. Spin-Ice State of the Quantum Heisenberg Antiferromagnet on the Pyrochlore Lattice.

    Science.gov (United States)

    Huang, Yuan; Chen, Kun; Deng, Youjin; Prokof'ev, Nikolay; Svistunov, Boris

    2016-04-29

    We study the low-temperature physics of the SU(2)-symmetric spin-1/2 Heisenberg antiferromagnet on a pyrochlore lattice and find "fingerprint" evidence for the thermal spin-ice state in this frustrated quantum magnet. Our conclusions are based on the results of bold diagrammatic Monte Carlo simulations, with good convergence of the skeleton series down to the temperature T/J=1/6. The identification of the spin-ice state is done through a remarkably accurate microscopic correspondence for the static structure factor between the quantum Heisenberg, classical Heisenberg, and Ising models at all accessible temperatures, and the characteristic bowtie pattern with pinch points observed at T/J=1/6. The dynamic structure factor at real frequencies (obtained by the analytic continuation of numerical data) is consistent with diffusive spinon dynamics at the pinch points.

  16. Spin-Ice State of the Quantum Heisenberg Antiferromagnet on the Pyrochlore Lattice

    Science.gov (United States)

    Huang, Yuan; Chen, Kun; Deng, Youjin; Prokof'ev, Nikolay; Svistunov, Boris

    2016-04-01

    We study the low-temperature physics of the SU(2)-symmetric spin-1 /2 Heisenberg antiferromagnet on a pyrochlore lattice and find "fingerprint" evidence for the thermal spin-ice state in this frustrated quantum magnet. Our conclusions are based on the results of bold diagrammatic Monte Carlo simulations, with good convergence of the skeleton series down to the temperature T /J =1 /6 . The identification of the spin-ice state is done through a remarkably accurate microscopic correspondence for the static structure factor between the quantum Heisenberg, classical Heisenberg, and Ising models at all accessible temperatures, and the characteristic bowtie pattern with pinch points observed at T /J =1 /6 . The dynamic structure factor at real frequencies (obtained by the analytic continuation of numerical data) is consistent with diffusive spinon dynamics at the pinch points.

  17. Spin-resolved photoemission anti-ferromagnets : Direct observation of Zhang-Rice singlets in CuO

    NARCIS (Netherlands)

    Tjeng, LH; Sinkovic, B; Brookes, NB; Goedkoop, JB; Hesper, R; Pellegrin, E; deGroot, FMF; Altieri, S; Hulbert, SL; Shekel, E; Sawatzky, GA

    1997-01-01

    We demonstrate that it is possible to obtain spin-resolved valence band spectra with a very high degree of spin polarization from antiferromagnetic transition metal materials if the excitation light is circularly polarized and has an energy close to the cation 2p(3/2) (L(3)) white line. We are able

  18. Measuring spin correlations in optical lattices using superlattice potentials

    DEFF Research Database (Denmark)

    Pedersen, Kim Georg Lind; Andersen, Brian Møller; Bruun, Georg Morten;

    2011-01-01

    We suggest two experimental methods for probing both short- and long-range spin correlations of atoms in optical lattices using superlattice potentials. The first method involves an adiabatic doubling of the periodicity of the underlying lattice to probe neighboring singlet (triplet) correlations...... for fermions (bosons) by the occupation of the resulting vibrational ground state. The second method utilizes a time-dependent superlattice potential to generate spin-dependent transport by any number of prescribed lattice sites, and probes correlations by the resulting number of doubly occupied sites....... For experimentally relevant parameters, we demonstrate how both methods yield large signatures of antiferromagnetic correlations of strongly repulsive fermionic atoms in a single shot of the experiment. Lastly, we show how this method may also be applied to probe d-wave pairing, a possible ground-state candidate...

  19. Phase Diagram in a Random Mixture of Two Antiferromagnets with Competing Spin Anisotropies. I

    Science.gov (United States)

    Someya, Yoshiko

    1981-12-01

    The phase diagram of a random mixture of two antiferromagnets with competing spin anisotropies (A1-xBx) has been analyzed by extending the theory of Matsubara and Inawashiro, and Oguchi and Ishikawa. In the model assumed, the anisotropy energies are expressed by the anisotropic exchange interactions. According to this formulation, it has been shown that the concentration dependence of TN becomes a function of \\includegraphics{dummy.eps}, where P, Q=A, B; SP is a magnitude of P-spin, and JPQη is a η component of exchange integral between P- and Q-spin). Further, the phase boundary between an AF phase and an OAF (oblique antiferromagnetic) phase at T{=}0 K has been shown to be determined by α({\\equiv}SB/SA), if \\includegraphics{dummy.eps} are given. The obtained phase diagrams for Fe1-xCoxCl2, K2Mn1-xFexF4 and Fe1-xCoxCl2\\cdot2H2O are compared with the experimental ones.

  20. Spin-ordered ground state and thermodynamic behaviors of the spin-3/2 kagome Heisenberg antiferromagnet

    Science.gov (United States)

    Liu, Tao; Li, Wei; Su, Gang

    2016-09-01

    Three different tensor network (TN) optimization algorithms are employed to accurately determine the ground state and thermodynamic properties of the spin-3/2 kagome Heisenberg antiferromagnet. We found that the √{3 }×√{3 } state (i.e., the state with 120° spin configuration within a unit cell containing 9 sites) is the ground state of this system, and such an ordered state is melted at any finite temperature, thereby clarifying the existing experimental controversies. Three magnetization plateaus (m /ms=1 /3 ,23 /27 , and 25/27) were obtained, where the 1/3-magnetization plateau has been observed experimentally. The absence of a zero-magnetization plateau indicates a gapless spin excitation that is further supported by the thermodynamic asymptotic behaviors of the susceptibility and specific heat. At low temperatures, the specific heat is shown to exhibit a T2 behavior, and the susceptibility approaches a finite constant as T →0 . Our TN results of thermodynamic properties are compared with those from high-temperature series expansion. In addition, we disclose a quantum phase transition between q =0 state (i.e., the state with 120° spin configuration within a unit cell containing three sites) and √{3 }×√{3 } state in a spin-3/2 kagome XXZ model at the critical point Δc=0.54 . This study provides reliable and useful information for further explorations on high-spin kagome physics.

  1. Spin-spin correlations between two Kondo impurities coupled to an open Hubbard chain

    Science.gov (United States)

    Tiegel, A. C.; Dargel, P. E.; Hallberg, K. A.; Frahm, H.; Pruschke, T.

    2013-02-01

    In order to study the interplay between Kondo and Ruderman-Kittel-Kasuya-Yosida interaction, we calculate the spin-spin correlation functions between two Kondo impurities coupled to different sites of a half-filled open Hubbard chain. Using the density-matrix renormalization group (DMRG), we reexamine the exponents for the power-law decay of the correlation function between the two impurity spins as a function of the antiferromagnetic coupling J, the Hubbard interaction U, and the distance R between the impurities. The exponents for finite systems obtained in this work deviate from previously published DMRG calculations. We furthermore show that the long-distance behavior of the exponents is the same for impurities coupled to the bulk or to both ends of the chain. We note that a universal exponent for the asymptotic behavior can not be extracted from these finite-size systems with open boundary conditions.

  2. Elemental analysis and magnetism of hydronium jarosites-model kagome antiferromagnets and topological spin glasses

    Energy Technology Data Exchange (ETDEWEB)

    Wills, A S; Bisson, W G, E-mail: a.s.wills@ucl.ac.uk [Department of Chemistry, University College London, 20 Gordon Street, London WC1H 0AJ (United Kingdom)

    2011-04-27

    The jarosites are the most studied examples of kagome antiferromagnets. Research into them has inspired new directions in magnetism, such as the role of the Dzyaloshinsky-Moriya interaction in symmetry breaking, kagome spin ice, and whether spin glass-like phases can exist in the disorder-free limit. This last point is based around the observation of unconventional thermodynamic and kinetic responses in hydronium jarosite, H{sub 3}OFe{sub 3}(SO{sub 4}){sub 2}(OH){sub 6}, that have led to its classification as a 'topological' spin glass, reflecting the defining role that the underlying geometry of the kagome lattice plays in the formation of the spin glass state. In this paper we explore one of the fundamental questions concerning the frustrated magnetism in hydronium jarosite: whether the spin glass phase is the result of chemical disorder and concomitant randomness in the exchange interactions. Confirming previous crystallographic studies, we use elemental analysis to show that the nature of the low temperature magnetic state is not a simple function of chemical disorder and provide evidence to support the hypothesis that anisotropies drive the spin glass transition.

  3. Elemental analysis and magnetism of hydronium jarosites--model kagome antiferromagnets and topological spin glasses.

    Science.gov (United States)

    Wills, A S; Bisson, W G

    2011-04-27

    The jarosites are the most studied examples of kagome antiferromagnets. Research into them has inspired new directions in magnetism, such as the role of the Dzyaloshinsky-Moriya interaction in symmetry breaking, kagome spin ice, and whether spin glass-like phases can exist in the disorder-free limit. This last point is based around the observation of unconventional thermodynamic and kinetic responses in hydronium jarosite, H(3)OFe(3)(SO(4))(2)(OH)(6), that have led to its classification as a 'topological' spin glass, reflecting the defining role that the underlying geometry of the kagome lattice plays in the formation of the spin glass state. In this paper we explore one of the fundamental questions concerning the frustrated magnetism in hydronium jarosite: whether the spin glass phase is the result of chemical disorder and concomitant randomness in the exchange interactions. Confirming previous crystallographic studies, we use elemental analysis to show that the nature of the low temperature magnetic state is not a simple function of chemical disorder and provide evidence to support the hypothesis that anisotropies drive the spin glass transition.

  4. Spin-1/2 Heisenberg J1-J2 antiferromagnet on the kagome lattice

    Science.gov (United States)

    Iqbal, Yasir; Poilblanc, Didier; Becca, Federico

    2015-01-01

    We report variational Monte Carlo calculations for the spin-1/2 Heisenberg model on the kagome lattice in the presence of both nearest-neighbor J1 and next-nearest-neighbor J2 antiferromagnetic superexchange couplings. Our approach is based upon Gutzwiller projected fermionic states that represent a flexible tool to describe quantum spin liquids with different properties (e.g., gapless and gapped). We show that, on finite clusters, a gapped Z2 spin liquid can be stabilized in the presence of a finite J2 superexchange, with a substantial energy gain with respect to the gapless U (1 ) Dirac spin liquid. However, this energy gain vanishes in the thermodynamic limit, implying that, at least within this approach, the U (1 ) Dirac spin liquid remains stable in a relatively large region of the phase diagram. For J2/J1≳0.3 , we find that a magnetically ordered state with q =0 overcomes the magnetically disordered wave functions, suggesting the end of the putative gapless spin-liquid phase.

  5. Specific Heat of the Spin-1/2 Antiferromagnetic Heisenberg Chain

    Institute of Scientific and Technical Information of China (English)

    云国宏; 梁希侠

    2001-01-01

    A simple analytic theory of thermodynamics at finite temperature for the spin-1/2 antiferromagnetic Heisenberg chain is proposed based on the picture of the particle-hole pair excitations. The dispersion relation of the particle-hole pairs is derived in the formulation of thermodynamic Bethe ansatz provided that the particles and holes have the same energy and they are excited as normalmodes. It is shown that the behaviour of the specific heat is in excellent agreement with the numerical and experimental results.

  6. Spin waves in a two-sublattice antiferromagnet. A self-similar solution of the Landau-Lifshitz equation

    Science.gov (United States)

    Gorobets, Y. I.; Gorobets, Y.; Kulish, V. V.

    2017-01-01

    In the paper, spin waves in a uniaxial two-sublattice antiferromagnet are investigated. A new class of self-similar solutions of the Landau-Lifshitz equation is obtained and, therefore, a new type of spin waves is described. Examples of solutions of the found class are presented. New type of solution admits both linear and non-linear spin waves, including solitons. Space transformations used in the solution are mathematically analogous to the relativistic transformations.

  7. Superconductivity, antiferromagnetism, and neutron scattering

    Science.gov (United States)

    Tranquada, John M.; Xu, Guangyong; Zaliznyak, Igor A.

    2014-01-01

    High-temperature superconductivity in both the copper-oxide and the iron-pnictide/chalcogenide systems occurs in close proximity to antiferromagnetically ordered states. Neutron scattering has been an essential technique for characterizing the spin correlations in the antiferromagnetic phases and for demonstrating how the spin fluctuations persist in the superconductors. While the nature of the spin correlations in the superconductors remains controversial, the neutron scattering measurements of magnetic excitations over broad ranges of energy and momentum transfers provide important constraints on the theoretical options. We present an overview of the neutron scattering work on high-temperature superconductors and discuss some of the outstanding issues.

  8. Padé approximations for the magnetic susceptibilities of Heisenberg antiferromagnetic spin chains for various spin values.

    Science.gov (United States)

    Law, J M; Benner, H; Kremer, R K

    2013-02-13

    The temperature dependence of the spin susceptibilities of S = 1, 3/2, 2, 5/2 and 7/2 Heisenberg antiferromagnetic 1D spins chains with nearest-neighbor coupling was simulated via quantum Monte Carlo calculations, within the reduced temperature range of 0.005 ≤ T* ≤ 100, and fitted to a Padé approximation with deviations between the simulated and fitted data of the same order of magnitude as or smaller than the quantum Monte Carlo simulation error. To demonstrate the practicality of our theoretical findings, we compare these results with the susceptibility of the well known 1D chain compound TMMC ([(CH(3))(4)N[MnCl(3)

  9. Disorder effects in the S=1 antiferromagnetic spin ladder CaV{sub 2}O{sub 4}

    Energy Technology Data Exchange (ETDEWEB)

    Guitarra, S.R. [Colegio de Ciencias e Ingeniería, Universidad San Francisco de Quito, Quito (Ecuador); Caneiro, A. [Instituto Balseiro - Centro Atómico Bariloche, 8400 Bariloche (Argentina); Niebieskikwiat, D., E-mail: dniebieskikwiat@usfq.edu.ec [Colegio de Ciencias e Ingeniería, Universidad San Francisco de Quito, Quito (Ecuador)

    2015-10-15

    We study the physical properties of the antiferromagnetic spin ladder CaV{sub 2}O{sub 4} (CVO) and the Y-doped related compound Ca{sub 0.9}Y{sub 0.1}V{sub 2}O{sub 4}. In the latter, X-ray diffraction demonstrates the segregation of a small amount of a vanadium–perovskite impurity phase, leading to the formation of V vacancies within the main CVO-type structure. The 1D character of this calcium–vanadite enhances the influence of the vacancies on the electric and magnetic properties of Ca{sub 0.9}Y{sub 0.1}V{sub 2}O{sub 4}. Electrical transport is characterized by a variable-range hopping mechanism determined by the charging energy of nm-sized segments of V chains delimited by V vacancies, i.e. a Coulomb gap is formed at the Fermi level. These vacancies also locally affect the magnetic correlations, breaking the long-range AFM order observed in CaV{sub 2}O{sub 4} and producing exchange bias when the Y-doped sample is cooled with an applied magnetic field. - Highlights: • We study disorder effects in the quasi-1D antiferromagnetic spin ladder CaV{sub 2}O{sub 4}. • V vacancies in CaV{sub 2}O{sub 4} lead to variable-range hopping electrical transport. • The charging energy of nm-sized V chains determine the transport mechanism exponents. • V vacancies break the long-range AFM order of CaV{sub 2}O{sub 4}. • Local magnetic correlations in the vicinity of the defects produce exchange bias.

  10. Studies on a frustrated Heisenberg spin chain with alternating ferromagnetic and antiferromagnetic exchanges.

    Science.gov (United States)

    Sahoo, Shaon; Durga Prasad Goli, V M L; Sen, Diptiman; Ramasesha, S

    2014-07-09

    We study Heisenberg spin-1/2 and spin-1 chains with alternating ferromagnetic (J(F)(1)) and antiferromagnetic (J(A)(1)) nearest-neighbor interactions and a ferromagnetic next-nearest-neighbor interaction (J(F)(2)). In this model frustration is present due to the non-zero J(F)(2). The model with site spin s behaves like a Haldane spin chain, with site spin 2s in the limit of vanishing J(F)(2)and large J(F)(1)/J(A)(1). We show that the exact ground state of the model can be found along a line in the parameter space. For fixed J(F)(1), the phase diagram in the space of J(A)(1)-J(F)(2) is determined using numerical techniques complemented by analytical calculations. A number of quantities, including the structure factor, energy gap, entanglement entropy and zero temperature magnetization, are studied to understand the complete phase diagram. An interesting and potentially important feature of this model is that it can exhibit a macroscopic magnetization jump in the presence of a magnetic field; we study this using an effective Hamiltonian.

  11. Electrical switching of antiferromagnets via strongly spin-orbit coupled materials

    Science.gov (United States)

    Li, Xi-Lai; Duan, Xiaopeng; Semenov, Yuriy G.; Kim, Ki Wook

    2017-01-01

    Electrically controlled ultra-fast switching of an antiferromagnet (AFM) is shown to be realizable by interfacing it with a material of strong spin-orbit coupling. The proximity interaction between the sublattice magnetic moments of a layered AFM and the spin-polarized free electrons at the interface offers an efficient way to manipulate antiferromagnetic states. A quantitative analysis, using the combination with a topological insulator as an example, demonstrates highly reliable 90° and 180° rotations of AFM magnetic states under two different mechanisms of effective torque generation at the interface. The estimated switching speed and energy requirement are in the ps and aJ ranges, respectively, which are about two-three orders of magnitude better than the ferromagnetic counterparts. The observed differences in the magnetization dynamics may explain the disparate characteristic responses. Unlike the usual precessional/chiral motions in the ferromagnets, those of the AFMs can essentially be described as a damped oscillator with a more direct path. The impact of random thermal fluctuations is also examined.

  12. Magnetization switching by spin-orbit torque in an antiferromagnet-ferromagnet bilayer system

    Science.gov (United States)

    Fukami, Shunsuke; Zhang, Chaoliang; Duttagupta, Samik; Kurenkov, Aleksandr; Ohno, Hideo

    2016-05-01

    Spin-orbit torque (SOT)-induced magnetization switching shows promise for realizing ultrafast and reliable spintronics devices. Bipolar switching of the perpendicular magnetization by the SOT is achieved under an in-plane magnetic field collinear with an applied current. Typical structures studied so far comprise a nonmagnet/ferromagnet (NM/FM) bilayer, where the spin Hall effect in the NM is responsible for the switching. Here we show that an antiferromagnet/ferromagnet (AFM/FM) bilayer system also exhibits a SOT large enough to switch the magnetization of the FM. In this material system, thanks to the exchange bias of the AFM, we observe the switching in the absence of an applied field by using an antiferromagnetic PtMn and ferromagnetic Co/Ni multilayer with a perpendicular easy axis. Furthermore, tailoring the stack achieves a memristor-like behaviour where a portion of the reversed magnetization can be controlled in an analogue manner. The AFM/FM system is thus a promising building block for SOT devices as well as providing an attractive pathway towards neuromorphic computing.

  13. Dilution Effects on Two-Dimensional Heisenberg Antiferromagnets with Non-Magnetic Spin-Gapped Ground State

    OpenAIRE

    Yasuda, Chitoshi; Todo, Synge; Matsumoto, Munehisa; Takayama, Hajime

    2002-01-01

    Dilution effects on spin-1/2 quantum Heisenberg antiferromagnets with a non-magnetic spin-gapped ground state are studied by means of the qunatum Monte Carlo simulation. In the site-diluted system, an antiferromagnetic long-range order (AF-LRO) is induced at an infinitesimal concentration of dilution due to an effective coupling $\\tilde{J}_{mn}$ between induced magnetic moments. In the bond-diluted case, on the other hand, the AF-LRO is not induced up to a certain concentration of dilution du...

  14. Longitudinal optical and spin Hall conductivities of Rashba conducting strips coupled to ferromagnetic and antiferromagnetic layers

    Science.gov (United States)

    Riera, José A.

    2017-01-01

    A system composed of a conducting planar strip with Rashba spin-orbit coupling (RSOC), magnetically coupled to a layer of localized magnetic moments, at equilibrium, is studied within a microscopic Hamiltonian with numerical techniques at zero temperature in the clean limit. In particular, transport properties for the cases of ferromagnetic (FM) and antiferromagnetic (AFM) coupled layers are computed in linear response on strips of varying width. Some behaviors observed for these properties are consistent with the ones observed for the corresponding Rashba helical currents. The case of uncoupled Rashba strips is also studied for comparison. In the case of Rashba strips coupled to an AFM localized order, results for the longitudinal dc conductivity, for small strip widths, suggest the proximity to a metal-insulator transition. More interesting, in the proximity of this transition, and in general at intermediate values of the RSOC, a large spin Hall conductivity is observed that is two orders of magnitude larger than the one for the FM order for the same values of the RSOC and strip widths. There are clearly two different regimes for small and for large RSOC, which is also present in the behavior of Rashba helical currents. Different contributions to the optical and the spin Hall conductivities, according to a new classification of inter- or intraband origin proposed for planar strips in the clean limit, or coming from the hopping or spin-orbit terms of the Hamiltonian, are examined. Finally, the effects of different orientation of the coupled magnetic moments will be also studied.

  15. Search for the Heisenberg spin glass on rewired cubic lattices with antiferromagnetic interaction

    Science.gov (United States)

    Surungan, Tasrief

    2016-10-01

    Spin glass (SG) is a typical magnetic system which is mainly characterized by a frozen random spin orientation at low temperatures. Frustration and randomness are considered to be the key ingredients for the existence of SGs. Previously, Bartolozzi et al. [Phys. Rev. B73, 224419 (2006)] found that the antiferromagnetic (AF) Ising spins on scale free network (SFN) exhibited SG behavior. This is purely AF system, a new type of SG different from the canonical one which requires the presence of both FM and AF couplings. In this new system, frustration is purely due to a topological factor and its randomness is brought by irregular connectivity. Recently, it was reported that the AF Heisenberg model on SFN exhibited SG behavior [Surungan et al., JPCS, 640, 012005 (2015)/doi:10.1088/1742-6596/640/1/012005]. In order to accommodate the notion of spatial dimension, we further investigated this type of system by studying an AF Heisenberg model on rewired cubic lattices, constructed by adding one extra bond randomly connecting each spin to one of its next-nearest neighbors. We used Replica Exchange algorithm of Monte Carlo Method and calculated the SG order parameter to search for the existence of SG phase.

  16. Charge stripes and spin correlations in copper-oxide superconductors

    Energy Technology Data Exchange (ETDEWEB)

    Tranquada, J.M.

    1997-05-01

    To obtain superconductivity in a layered copper-oxide compound, it is necessary to introduce charge carriers into the antiferromagnetic CuO{sub 2} planes. Recent neutron diffraction studies of the system La{sub 1.6-x}Nd{sub 0.4}Sr{sub x}CuO{sub 4} provide evidence that the dopant-induced holes choose to segregate into periodically-spaced stripes which separate antiferromagnetic domains, in a manner similar to that found in hole-doped La{sub 2}NiO{sub 4}. The charge and spin stripe modulations are identified by the appearance of scattering at incommensurate positions. In the Nd-doped system, elastic scattering is observed, corresponding to static stripes. In pure La{sub 2-x}Sr{sub x}CuO{sub 4}, the magnetic scattering that is observed is purely inelastic. Where samples with and without Nd, but with the same Sr concentration, have been measured, the incommensurate (IC) splittings of the magnetic signal are found to be essentially identical. It has been proposed that the spin correlations in the two systems are fundamentally the same, thus implying similar charge correlations. The static nature of the stripes in the Nd-doped system is attributed to pinning of the otherwise dynamic correlations by a special distortion of the lattice. That distortion is driven by purely ionic interactions and is stabilized by the smaller ionic radius of the substituted Nd.

  17. Magnetic structure and spin dynamics of the quasi-one-dimensional spin-chain antiferromagnet BaCo2V2O8

    DEFF Research Database (Denmark)

    Kawasaki, Yu; Gavilano, Jorge L.; Keller, Lukas

    2011-01-01

    We report a neutron diffraction and muon spin relaxation mu SR study of static and dynamical magnetic properties of BaCo2V2O8, a quasi-one-dimensional spin-chain system. A proposed model for the antiferromagnetic structure includes: a propagation vector (k) over right arrow (AF) = (0,0,1), indepe......We report a neutron diffraction and muon spin relaxation mu SR study of static and dynamical magnetic properties of BaCo2V2O8, a quasi-one-dimensional spin-chain system. A proposed model for the antiferromagnetic structure includes: a propagation vector (k) over right arrow (AF) = (0...... at different muon stopping sites. Muon time spectra measured at weak longitudinal fields and temperatures much higher than T-N can be well described using a single muon site with an exponential muon spin relaxation that gradually changes into an stretched exponential on approaching T-N. The temperature...

  18. Low temperature ballistic spin transport in the S = 1/2 antiferromagnetic Heisenberg chain compound SrCuO2.

    Science.gov (United States)

    Maeter, H; Zvyagin, A A; Luetkens, H; Pascua, G; Shermadini, Z; Saint-Martin, R; Revcolevschi, A; Hess, C; Büchner, B; Klauss, H-H

    2013-09-11

    We report zero and longitudinal magnetic field muon spin relaxation (μSR) measurements of the spin S = 1/2 antiferromagnetic Heisenberg chain material SrCuO2. We find that in a weak applied magnetic field B0 the spin-lattice relaxation rate λ follows a power law λ is proportional to B(0)(-n) with n = 0.9(3). This result is temperature independent for 5 K ≤ T ≤ 300 K. Within conformal field theory and using the Müller ansatz we conclude ballistic spin transport in SrCuO2.

  19. Characterization of Topological Phases of Spin-1/2 Frustrated Ferromagnetic-Antiferromagnetic Alternating Heisenberg Chains by Entanglement Spectrum

    Science.gov (United States)

    Hida, Kazuo

    2016-02-01

    The topological classification of a series of frustration-induced spin-gap phases in the spin-1/2 ferromagnetic-antiferromagnetic alternating Heisenberg chain with next-nearest-neighbour interaction reported in J. Phys. Soc. Jpn. 82, 064703 (2013) is confirmed using two kinds of entanglement spectra defined by different divisions of the whole chain. For the numerical calculation, the iDMRG method is used. The results are consistent with the valence bond solid picture proposed in the previous paper.

  20. Coordinate Bethe ansatz computation for low temperature behavior of a triangular lattice of a spin-1 Heisenberg antiferromagnet

    Energy Technology Data Exchange (ETDEWEB)

    Shuaibu, A. [Department of Physics, Faculty of Science, Universiti Putra Malaysia, 43400 UPM Serdang, Selangor, Malaysia and Physics Department, Faculty of Science, Nigerian Defence Academy, P.M.B 2109, Kaduna (Nigeria); Rahman, M. M. [Physics Department, Faculty of Science, Nigerian Defence Academy, P.M.B 2109, Kaduna (Nigeria)

    2014-03-05

    We study the low temperature behavior of a triangular lattice quantum spin-1 Heisenberg antiferromagnet with single-site anisotropy by using coordinate Bethe ansatz method. We compute the standard two-particle Hermitian Hamiltonian, and obtain the eigenfunctions and eigenvalue of the system. The obtained results show a number of advantages in comparison with many results.

  1. Spin liquid in a single crystal of the frustrated diamond lattice antiferromagnet CoAl2O4

    DEFF Research Database (Denmark)

    Zaharko, O.; Christensen, Niels Bech; Cervellino, A.

    2011-01-01

    We study the evidence for spin liquid in the frustrated diamond lattice antiferromagnet CoAl2O4 by means of single-crystal neutron scattering in zero and applied magnetic fields. The magnetically ordered phase appearing below T-N = 8 K remains nonconventional down to 1.5 K. The magnetic Bragg peaks...

  2. Role of the antiferromagnetic pinning layer on spin wave properties in IrMn/NiFe based spin-valves

    Energy Technology Data Exchange (ETDEWEB)

    Gubbiotti, G., E-mail: gubbiotti@fisica.unipg.it; Tacchi, S. [Istituto Officina dei Materiali del CNR (IOM-CNR), Unità di Perugia, I-06123 Perugia (Italy); Del Bianco, L. [Department of Physics and Astronomy, University of Bologna, I-40127 Bologna (Italy); Department of Physics and Earth Sciences and CNISM, University of Ferrara, I-44122 Ferrara (Italy); Bonfiglioli, E.; Giovannini, L.; Spizzo, F.; Zivieri, R. [Department of Physics and Earth Sciences and CNISM, University of Ferrara, I-44122 Ferrara (Italy); Tamisari, M. [Department of Physics and Earth Sciences and CNISM, University of Ferrara, I-44122 Ferrara (Italy); Dipartimento di Fisica e Geologia, Università di Perugia, I-06123 Perugia (Italy)

    2015-05-07

    Brillouin light scattering (BLS) was exploited to study the spin wave properties of spin-valve (SV) type samples basically consisting of two 5 nm-thick NiFe layers (separated by a Cu spacer of 5 nm), differently biased through the interface exchange coupling with an antiferromagnetic IrMn layer. Three samples were investigated: a reference SV sample, without IrMn (reference); one sample with an IrMn underlayer (10 nm thick) coupled to the bottom NiFe film; one sample with IrMn underlayer and overlayer of different thickness (10 nm and 6 nm), coupled to the bottom and top NiFe film, respectively. The exchange coupling with the IrMn, causing the insurgence of the exchange bias effect, allowed the relative orientation of the NiFe magnetization vectors to be controlled by an external magnetic field, as assessed through hysteresis loop measurements by magneto-optic magnetometry. Thus, BLS spectra were acquired by sweeping the magnetic field so as to encompass both the parallel and antiparallel alignment of the NiFe layers. The BLS results, well reproduced by the presented theoretical model, clearly revealed the combined effects on the spin dynamic properties of the dipolar interaction between the two NiFe films and of the interface IrMn/NiFe exchange coupling.

  3. Glass-like recovery of antiferromagnetic spin ordering in a photo-excited manganite Pr0.7Ca0.3MnO3

    Energy Technology Data Exchange (ETDEWEB)

    Zhou, S. Y.; Langner, M. C.; Zhu, Y.; Chuang, Y. -D.; Rini, M.; Glover, T. E.; Hertlein, M. P.; Gonzalez, A.G. Cruz; Tahir, N.; Tomioka, Y.; Tokura, Y.; Hussain, Z.; Schoenlein, R. W.

    2014-01-16

    Electronic orderings of charges, orbitals and spins are observed in many strongly correlated electron materials, and revealing their dynamics is a critical step toward understanding the underlying physics of important emergent phenomena. Here we use time-resolved resonant soft x-ray scattering spectroscopy to probe the dynamics of antiferromagnetic spin ordering in the manganite Pr0:7Ca0:3MnO3 following ultrafast photo-exitation. Our studies reveal a glass-like recovery of the spin ordering and a crossover in the dimensionality of the restoring interaction from quasi-1D at low pump fluence to 3D at high pump fluence. This behavior arises from the metastable state created by photo-excitation, a state characterized by spin disordered metallic droplets within the larger charge- and spin-ordered insulating domains. Comparison with time-resolved resistivity measurements suggests that the collapse of spin ordering is correlated with the insulator-to-metal transition, but the recovery of the insulating phase does not depend on the re-establishment of the spin ordering.

  4. Spin dynamics of S = 1/2 kagome lattice antiferromagnets observed by high-field ESR

    Energy Technology Data Exchange (ETDEWEB)

    Ohta, Hitoshi [Molecular Photoscience Research Center, Kobe University, Kobe 657-8501 (Japan); Graduate School of Science, Kobe University, Kobe 657-8501 (Japan); Zhang, Wei-min [Graduate School of Science, Kobe University, Kobe 657-8501 (Japan); Okubo, Susumu; Fujisawa, Masashi [Molecular Photoscience Research Center, Kobe University, Kobe 657-8501 (Japan); Sakurai, Takahiro [Center for Supports to Research and Education Activities, Kobe University, Kobe 657-8501 (Japan); Okamoto, Yoshihiko; Yoshida, Hiroyuki; Hiroi, Zenji [Institute for Solid State Physics (ISSP), University of Tokyo, Kashiwa, Chiba 277-8581 (Japan)

    2010-03-15

    Due to the existence of strong spin frustration in a system, the spin dynamics of S = 1/2 kagome lattice antiferromagnet at low temperature has attracted much interest. High-field ESR has been measured on its model substances, Cu{sub 3}V{sub 2}O{sub 7}(OH){sub 2} . 2H{sub 2}O (volborthite) and BaCu{sub 3}V{sub 2}O{sub 3}(OH){sub 2} (vesignieite), down to 1.8 K using pulsed magnetic fields up to 16 T. The measurements are performed for 160 and 315 GHz using polycrys-talline samples. Although both samples showed the g-shift and the change of linewidth at low temperature, volborthite showed a small gap excitation of the order of 40 GHz (1.9 K) while vesignieite showed a paramagnetic behavior down to 1.9 K. Observed difference will be discussed in connection with the crystal structure, and the possible spin liquid state in vesignieite will be discussed. (Abstract Copyright [2010], Wiley Periodicals, Inc.)

  5. Search for the Heisenberg spin glass on rewired square lattices with antiferromagnetic interaction

    Science.gov (United States)

    Surungan, Tasrief; Bansawang B., J.; Tahir, Dahlang

    2016-03-01

    Spin glass (SG) is a typical magnetic system with frozen random spin orientation at low temperatures. The system exhibits rich physical properties, such as infinite number of ground states, memory effect, and aging phenomena. There are two main ingredients considered to be pivotal for the existence of SG behavior, namely, frustration and randomness. For the canonical SG system, frustration is led by the presence of competing interaction between ferromagnetic (FM) and antiferromagnetic (AF) couplings. Previously, Bartolozzi et al. [Phys. Rev. B73, 224419 (2006)], reported the SG properties of the AF Ising spins on scale free network (SFN). It is a new type of SG, different from the canonical one which requires the presence of both FM and AF couplings. In this new system, frustration is purely caused by the topological factor and its randomness is related to the irregular connectvity. Recently, Surungan et. al. [Journal of Physics: Conference Series, 640, 012001 (2015)] reported SG bahavior of AF Heisenberg model on SFN. We further investigate this type of system by studying an AF Heisenberg model on rewired square lattices. We used Replica Exchange algorithm of Monte Carlo Method and calculated the SG order parameter to search for the existence of SG phase.

  6. Two-dimensional-lattice spin models with long-range antiferromagnetic interactions

    Science.gov (United States)

    Romano, S.

    1991-10-01

    We consider a classical system, consisting of m-component unit vectors (m=2,3), associated with a two-dimensional lattice \\{uk||k∈openZ2\\} and interacting via translationally and rotationally invariant antiferromagnetic pair potentials of the long-range form W=Wjk=ɛ||xj-xk||-puj.uk, p>2, where ɛ is a positive quantity, setting energy and temperature scales (i.e., T*=kBT/ɛ), and xk are the coordinates of the lattice sites. A spin-wave approach predicts orientational disorder (in the thermodynamic limit) at all finite temperatures and for all p>2 this agrees with available rigorous results for p>=4, whereas no such theorems are known in the literature when 22.

  7. A separation of antiferromagnetic spin motion modes in the training effect of exchange biased Co/CoO film with in-plane anisotropy

    Science.gov (United States)

    Wu, R.; Yun, C.; Ding, S. L.; Wen, X.; Liu, S. Q.; Wang, C. S.; Han, J. Z.; Du, H. L.; Yang, J. B.

    2016-08-01

    The motion of antiferromagnetic interfacial spins is investigated through the temperature evolution of training effect in a Co/CoO film with in-plane biaxial anisotropy. Significant differences in the training effect and its temperature dependence are observed in the magnetic easy axis and hard axis (HA) and ascribed to the different motion modes of antiferromagnetic interfacial spins, the collective spin cluster rotation (CSR) and the single spin reversal (SSR), caused by different magnetization reversal modes of ferromagnetic layer. These motion modes of antiferromagnetic spins are successfully separated using a combination of an exponential function and a classic n-1/2 function. A larger CSR to SSR ratio and a shorter lifetime of CSR found in the HA indicates that the domain rotation in the ferromagnetic layer tends to activate and accelerate a CSR mode in the antiferromagnetic spins.

  8. Probing ultrafast spin dynamics through a magnon resonance in the antiferromagnetic multiferroic HoMnO3

    Science.gov (United States)

    Bowlan, P.; Trugman, S. A.; Bowlan, J.; Zhu, J.-X.; Hur, N. J.; Taylor, A. J.; Yarotski, D. A.; Prasankumar, R. P.

    2016-09-01

    We demonstrate an approach for directly tracking antiferromagnetic (AFM) spin dynamics by measuring ultrafast changes in a magnon resonance. We test this idea on the multiferroic HoMnO3 by optically photoexciting electrons, after which changes in the spin order are probed with a THz pulse tuned to a magnon resonance. This reveals a photoinduced change in the magnon line shape that builds up over 5-12 picoseconds, which we show to be the spin-lattice thermalization time, indicating that electrons heat the spins via phonons. We compare our results to previous studies of spin-lattice thermalization in ferromagnetic manganites, giving insight into fundamental differences between the two systems. Our work sheds light on the microscopic mechanism governing spin-phonon interactions in AFMs and demonstrates a powerful approach for directly monitoring ultrafast spin dynamics.

  9. Top Quark Spin Correlations at the Tevatron

    Energy Technology Data Exchange (ETDEWEB)

    Head, Tim; /Manchester U.

    2010-07-01

    Recent measurements of the correlation between the spin of the top and the spin of the anti-top quark produced in proton anti-proton scattering at a center of mass energy of {radical}s = 1.96 Tev by the CDF and D0 collaborations are discussed. using up to 4.3 fb{sup -1} of data taken with the CDF and D0 detectors the spin correlation parameter C, the degree to which the spins are correlated, is measured in dileptonic and semileptonic final states. The measurements are found to be in agreement with Standard Model predictions.

  10. Correlated spin networks in frustrated systems

    Science.gov (United States)

    Stone, Thomas E.; McKay, Susan R.

    2010-08-01

    We introduce a network model for frustrated spin systems based on highly correlated spin fluctuations, to quantify and visualize their ordering. This model shows that networks of strongly correlated but non-contiguous spins exist at low temperatures on a triangular Ising lattice with competing nearest-neighbor interactions. This finding is consistent with chaotic renormalization-group trajectories previously reported for frustrated hierarchical lattices.

  11. Spin-glass transition in bond-disordered Heisenberg antiferromagnets coupled with local lattice distortions on a pyrochlore lattice.

    Science.gov (United States)

    Shinaoka, Hiroshi; Tomita, Yusuke; Motome, Yukitoshi

    2011-07-22

    Motivated by puzzling characteristics of spin-glass transitions widely observed in pyrochlore-based frustrated materials, we investigate the effects of coupling to local lattice distortions in a bond-disordered antiferromagnet on the pyrochlore lattice by extensive Monte Carlo simulations. We show that the spin-glass transition temperature T(f) is largely enhanced by the spin-lattice coupling and, furthermore, becomes almost independent of Δ in a wide range of the disorder strength Δ. The critical property of the spin-glass transition is indistinguishable from that of the canonical Heisenberg spin glass in the entire range of Δ. These peculiar behaviors are ascribed to a modification of the degenerate manifold from a continuous to semidiscrete one by spin-lattice coupling.

  12. Ultracold few fermionic atoms in needle-shaped double wells: spin chains and resonating spin clusters from microscopic Hamiltonians emulated via antiferromagnetic Heisenberg and t-J models

    Science.gov (United States)

    Yannouleas, Constantine; Brandt, Benedikt B.; Landman, Uzi

    2016-07-01

    Advances with trapped ultracold atoms intensified interest in simulating complex physical phenomena, including quantum magnetism and transitions from itinerant to non-itinerant behavior. Here we show formation of antiferromagnetic ground states of few ultracold fermionic atoms in single and double well (DW) traps, through microscopic Hamiltonian exact diagonalization for two DW arrangements: (i) two linearly oriented one-dimensional, 1D, wells, and (ii) two coupled parallel wells, forming a trap of two-dimensional, 2D, nature. The spectra and spin-resolved conditional probabilities reveal for both cases, under strong repulsion, atomic spatial localization at extemporaneously created sites, forming quantum molecular magnetic structures with non-itinerant character. These findings usher future theoretical and experimental explorations into the highly correlated behavior of ultracold strongly repelling fermionic atoms in higher dimensions, beyond the fermionization physics that is strictly applicable only in the 1D case. The results for four atoms are well described with finite Heisenberg spin-chain and cluster models. The numerical simulations of three fermionic atoms in symmetric DWs reveal the emergent appearance of coupled resonating 2D Heisenberg clusters, whose emulation requires the use of a t-J-like model, akin to that used in investigations of high T c superconductivity. The highly entangled states discovered in the microscopic and model calculations of controllably detuned, asymmetric, DWs suggest three-cold-atom DW quantum computing qubits.

  13. Antiferromagnetic THz-frequency Josephson-like Oscillator Driven by Spin Current

    Science.gov (United States)

    Khymyn, Roman; Lisenkov, Ivan; Tiberkevich, Vasyl; Ivanov, Boris A.; Slavin, Andrei

    2017-03-01

    The development of compact and tunable room temperature sources of coherent THz-frequency signals would open a way for numerous new applications. The existing approaches to THz-frequency generation based on superconductor Josephson junctions (JJ), free electron lasers, and quantum cascades require cryogenic temperatures or/and complex setups, preventing the miniaturization and wide use of these devices. We demonstrate theoretically that a bi-layer of a heavy metal (Pt) and a bi-axial antiferromagnetic (AFM) dielectric (NiO) can be a source of a coherent THz signal. A spin-current flowing from a DC-current-driven Pt layer and polarized along the hard AFM anisotropy axis excites a non-uniform in time precession of magnetizations sublattices in the AFM, due to the presence of a weak easy-plane AFM anisotropy. The frequency of the AFM oscillations varies in the range of 0.1–2.0 THz with the driving current in the Pt layer from 108 A/cm2 to 109 A/cm2. The THz-frequency signal from the AFM with the amplitude exceeding 1 V/cm is picked up by the inverse spin-Hall effect in Pt. The operation of a room-temperature AFM THz-frequency oscillator is similar to that of a cryogenic JJ oscillator, with the energy of the easy-plane magnetic anisotropy playing the role of the Josephson energy.

  14. Antiferromagnetic THz-frequency Josephson-like Oscillator Driven by Spin Current

    Science.gov (United States)

    Khymyn, Roman; Lisenkov, Ivan; Tiberkevich, Vasyl; Ivanov, Boris A.; Slavin, Andrei

    2017-01-01

    The development of compact and tunable room temperature sources of coherent THz-frequency signals would open a way for numerous new applications. The existing approaches to THz-frequency generation based on superconductor Josephson junctions (JJ), free electron lasers, and quantum cascades require cryogenic temperatures or/and complex setups, preventing the miniaturization and wide use of these devices. We demonstrate theoretically that a bi-layer of a heavy metal (Pt) and a bi-axial antiferromagnetic (AFM) dielectric (NiO) can be a source of a coherent THz signal. A spin-current flowing from a DC-current-driven Pt layer and polarized along the hard AFM anisotropy axis excites a non-uniform in time precession of magnetizations sublattices in the AFM, due to the presence of a weak easy-plane AFM anisotropy. The frequency of the AFM oscillations varies in the range of 0.1–2.0 THz with the driving current in the Pt layer from 108 A/cm2 to 109 A/cm2. The THz-frequency signal from the AFM with the amplitude exceeding 1 V/cm is picked up by the inverse spin-Hall effect in Pt. The operation of a room-temperature AFM THz-frequency oscillator is similar to that of a cryogenic JJ oscillator, with the energy of the easy-plane magnetic anisotropy playing the role of the Josephson energy. PMID:28262731

  15. Correlation functions of the antiferromagnetic Heisenberg model using a modified Lanczos method

    Science.gov (United States)

    Gagliano, Eduardo R.; Dagotto, Elbio; Moreo, Adriana; Alcaraz, Francisco C.

    1986-08-01

    Using a modified Lanczos algorithm, we study the correlation functions in the ground state of the one-dimensional antiferromagnetic Heisenberg model. We obtain numerical results for rings up to 24 sites. There are no indications of the anomalous behavior of these correlation functions recently observed in chains with 16 sites. We also present a pedagogical description of the hashing technique which is an efficient algorithm for searching and storage purposes.

  16. CP observables with spin spin correlations in chargino production

    Science.gov (United States)

    Bartl, A.; Hohenwarter-Sodek, K.; Kernreiter, T.; Kittel, O.; Terwort, M.

    2008-10-01

    We study the CP-violating terms of the spin-spin correlations in chargino production ee→χ˜1±χ˜2∓, and their subsequent two-body decays into sneutrinos plus leptons. We propose novel CP-sensitive observables with the help of T-odd products of the spin-spin terms. These terms depend on the polarizations of both charginos, with one polarization perpendicular to the production plane. We identify two classes of CP-sensitive observables; one requires the reconstruction of the production plane, the other not. Our framework is the Minimal Supersymmetric Standard Model with complex parameters.

  17. Refining the spin Hamiltonian in the spin-1/2 kagome lattice antiferromagnet ZnCu3(OH)6Cl2 using single crystals.

    Science.gov (United States)

    Han, Tianheng; Chu, Shaoyan; Lee, Young S

    2012-04-13

    We report thermodynamic measurements of the S=1/2 kagome lattice antiferromagnet ZnCu3(OH)6Cl2, a promising candidate system with a spin-liquid ground state. Using single crystal samples, the magnetic susceptibility both perpendicular and parallel to the kagome plane has been measured. A small, temperature-dependent anisotropy has been observed, where χ(z)/χ(p)>1 at high temperatures and χ(z)/χ(p)kagome Heisenberg antiferromagnet model to the experiments on ZnCu3(OH)6Cl2.

  18. Variational Monte Carlo study of a gapless spin liquid in the spin-1/2 XXZ antiferromagnetic model on the kagome lattice

    Science.gov (United States)

    Hu, Wen-Jun; Gong, Shou-Shu; Becca, Federico; Sheng, D. N.

    2015-11-01

    By using the variational Monte Carlo technique, we study the spin-1/2 XXZ antiferromagnetic model (with easy-plane anisotropy) on the kagome lattice. A class of Gutzwiller projected fermionic states with a spin Jastrow factor is considered to describe either spin liquids [with U (1 ) or Z2 symmetry] or magnetically ordered phases [with q =(0 ,0 ) or q =(4 π /3 ,0 ) ]. We find that the magnetic states are not stable in the thermodynamic limit. Moreover, there is no energy gain to break the gauge symmetry from U (1 ) to Z2 within the spin-liquid states, as previously found in the Heisenberg model. The best variational wave function is therefore the U (1 ) Dirac state, supplemented by the spin Jastrow factor. Furthermore, a vanishing S =2 spin gap is obtained at the variational level, in the whole regime from the X Y to the Heisenberg model.

  19. Spin-Hall-Effect-Assisted Electroresistance in Antiferromagnets via 105 A/cm2 dc Current

    Science.gov (United States)

    Han, Jiahao; Wang, Yuyan; Pan, Feng; Song, Cheng

    2016-08-01

    Antiferromagnet (AFM) spintronics with reduced electrical current is greatly expected to process information with high integration and low power consumption. In Pt/FeMn and Ta/FeMn hybrids, we observe significant resistance variation (up to 7% of the total resistance) manipulated by 105 A/cm2 dc current. We have excluded the contribution of isotropic structural effects, and confirmed the critical role of the spin Hall injection from Pt (or Ta) to FeMn. This electrical current-manipulated resistance (i.e. electroresistance) is proposed to be attributed to the spin-Hall-effect-induced spin-orbit torque in FeMn. Similar results have also been detected in plain IrMn films, where the charge current generates spin current via the spin Hall effect with the existence of Ir atoms. All the measurements are free from external magnetic fields and ferromagnets. Our findings present an interesting step towards high-efficiency spintronic devices.

  20. Spin dynamics and spin freezing in the triangular lattice antiferromagnets FeGa2S4 and NiGa2S4

    Science.gov (United States)

    Zhao, Songrui; Dalmas de Réotier, P.; Yaouanc, A.; MacLaughlin, D. E.; Mackie, J. M.; Bernal, O. O.; Nambu, Y.; Higo, T.; Nakatsuji, S.

    2012-08-01

    Magnetic susceptibility and muon spin relaxation (μSR) experiments have been carried out on the quasi-2D triangular-lattice spin S=2 antiferromagnet FeGa2S4. The μSR data indicate a sharp onset of a frozen or nearly frozen spin state at T*=31(2) K, twice the spin-glass-like freezing temperature Tf=16(1) K. The susceptibility becomes field dependent below T*, but no sharp anomaly is observed in any bulk property. A similar transition is observed in μSR data from the spin-1 isomorph NiGa2S4. In both compounds the dynamic muon spin relaxation rate λd(T) above T* agrees well with a calculation of spin-lattice relaxation by Chubukov, Sachdev, and Senthil in the renormalized classical regime of a 2D frustrated quantum antiferromagnet. There is no firm evidence for other mechanisms. At low temperatures, λd(T) becomes temperature independent in both compounds, indicating persistence of spin dynamics. Scaling of λd(T) between the two compounds is observed from ˜Tf to ˜1.5T*. Although the μSR data by themselves cannot exclude a truly static spin component below T*, together with the susceptibility data they are consistent with a slowly fluctuating “spin gel” regime between Tf and T*. Such a regime and the absence of a divergence in λd(T) at T* are features of two unconventional mechanisms: (1) binding/unbinding of Z2 vortex excitations, and (2) impurity spins in a nonmagnetic spin-nematic ground state. The absence of a sharp anomaly or history dependence at T* in the susceptibility of FeGa2S4, and the weakness of such phenomena in NiGa2S4, strongly suggest transitions to low-temperature phases with unconventional dynamics.

  1. Spin dynamics induced by ultrafast heating with ferromagnetic/antiferromagnetic interfacial exchange in perpendicularly magnetized hard/soft bilayers

    Energy Technology Data Exchange (ETDEWEB)

    Ma, Q. L., E-mail: maqinli@gmail.com, E-mail: mizukami@wpi-aimr.tohoku.ac.jp; Miyazaki, T.; Mizukami, S., E-mail: maqinli@gmail.com, E-mail: mizukami@wpi-aimr.tohoku.ac.jp [WPI Advanced Institute for Materials Research, Tohoku University, 2-1-1, Katahira, 980-8577 Sendai (Japan); Iihama, S. [Department of Applied Physics, Tohoku University, 6-6-05 Aza-Aoba, Aramaki, Aoba-ku, Sendai 980-8579 (Japan); Zhang, X. M. [Key Laboratory for Anisotropy and Texture of Materials, Ministry of Education, Northeastern University, Shenyang 110819 (China)

    2015-11-30

    The laser-induced spin dynamics of FeCo in perpendicularly magnetized L1{sub 0}-MnGa/FeCo bilayers with ferromagnetic and antiferromagnetic interfacial exchange coupling (IEC) are examined using the time-resolved magneto-optical Kerr effect. We found a precessional phase reversal of the FeCo layer as the IEC changes from ferromagnetic to antiferromagnetic. Moreover, a precession-suspension window was observed when the magnetic field was applied in a certain direction for the bilayer with ferromagnetic IEC. Our observations reveal that the spin dynamics modulation is strongly dependent on the IEC type within the Landau-Lifshitz-Gilbert depiction. The IEC dependence of the precessional phase and amplitude suggests the interesting method for magnetization dynamics modulation.

  2. Antiferromagnetic versus spin-glass like behavior in MnIn{sub 2}S{sub 4}

    Energy Technology Data Exchange (ETDEWEB)

    Sagredo, V. [Laboratorio de Magnetismo, Departamento de Fisica, Facultad de Ciencias, Universidad de los Andes, Merida (Venezuela)]. E-mail: sagredo@ula.ve; Moron, M.C. [Instituto de Ciencia de Materiales de Aragon, C.S.I.C.-Universidad de Zaragoza, E-50009, Zaragoza (Spain); Betancourt, L. [Laboratorio de Magnetismo, Departamento de Fisica, Facultad de Ciencias, Universidad de los Andes, Merida (Venezuela); Delgado, G.E. [Laboratorio de Cristalografia, Departamento de Quimica, Facultad de Ciencias, Universidad de los Andes, Merida (Venezuela)

    2007-05-15

    The low-temperature magnetic properties of MnIn{sub 2}S{sub 4} have been studied using AC magnetic susceptibility and magnetization experiments. High-temperature susceptibility fits indicate the presence of antiferromagnetic interactions. Low-field magnetization data show a peak at 5.6{+-}0.1 K, below which strong irreversibility is observed between zero-field-cooled (ZFC) and field-cooled (FC) cycles suggesting that the observed peak corresponds to a spin-glass-like transition instead of the antiferromagnetic one previously reported. Further evidence of this magnetic state comes from AC susceptibility data at different frequencies. The in-phase component {chi}'(T) exhibits the behavior expected of spin glasses, i.e. a shift of the cusp to higher temperatures for higher frequencies.

  3. Cu, Pu and Fe high T{sub c} superconductors: Spin holes in anti-ferromagnetic clusters form nonmagnetic bipolarons

    Energy Technology Data Exchange (ETDEWEB)

    Wachter, Peter, E-mail: wachter@solid.phys.ethz.c [Laboratorium fuer Festkoerperphysik, ETH Zuerich, 8093 Zuerich (Switzerland)

    2009-03-15

    The new iron based high T{sub c} superconductors with T{sub c} up to 55 K have stirred new interest in this field. It is consensus that the BCS mechanism is not able to explain the high T{sub c}'s. In the following we propose that spin holes in anti-ferromagnetic clusters combine to make nonmagnetic bipolarons, which can condense and lead to superconductivity.

  4. Spin glass behavior of the antiferromagnetic Heisenberg model on scale free network

    Science.gov (United States)

    Surungan, Tasrief; Zen, Freddy P.; Williams, Anthony G.

    2015-09-01

    Randomness and frustration are considered to be the key ingredients for the existence of spin glass (SG) phase. In a canonical system, these ingredients are realized by the random mixture of ferromagnetic (FM) and antiferromagnetic (AF) couplings. The study by Bartolozzi et al. [Phys. Rev. B73, 224419 (2006)] who observed the presence of SG phase on the AF Ising model on scale free network (SFN) is stimulating. It is a new type of SG system where randomness and frustration are not caused by the presence of FM and AF couplings. To further elaborate this type of system, here we study Heisenberg model on AF SFN and search for the SG phase. The canonical SG Heisenberg model is not observed in d-dimensional regular lattices for (d ≤ 3). We can make an analogy for the connectivity density (m) of SFN with the dimensionality of the regular lattice. It should be plausible to find the critical value of m for the existence of SG behaviour, analogous to the lower critical dimension (dl) for the canonical SG systems. Here we study system with m = 2, 3, 4 and 5. We used Replica Exchange algorithm of Monte Carlo Method and calculated the SG order parameter. We observed SG phase for each value of m and estimated its corersponding critical temperature.

  5. Approximation algorithms for two-state anti-ferromagnetic spin systems on bounded degree graphs

    CERN Document Server

    Sinclair, Alistair; Thurley, Marc

    2011-01-01

    In a seminal paper (Weitz, 2006), Weitz gave a deterministic fully polynomial approximation scheme for counting exponentially weighted independent sets (which is the same as approximating the partition function of the hard-core model from statistical physics) in graphs of degree at most d, up to the critical activity for the uniqueness of the Gibbs measure on the infinite d-regular tree. More recently Sly (see also Galanis et al, 2011) showed that this is optimal in the sense that if there is an FPRAS for the hard-core partition function on graphs of maximum degree d for activities larger than the critical activity on the infinite d-regular tree then NP = RP. In this paper we extend Weitz's approach to derive a deterministic fully polynomial approximation scheme for the partition function of general two-state anti-ferromagnetic spin systems on graphs of maximum degree d, up to the corresponding critical point on the d-regular tree. The main ingredient of our result is a proof that for two-state anti-ferromagn...

  6. Coexistence of antiferromagnetic and ferromagnetic spin correlations in Ca(Fe1-xCox)2As2 revealed by As75 nuclear magnetic resonance

    Energy Technology Data Exchange (ETDEWEB)

    Cui, J.; Wiecki, P.; Ran, S.; Bud' ko, S. L.; Canfield, P. C.; Furukawa, Y.

    2016-11-22

    Recent nuclear magnetic resonance (NMR) measurements revealed the coexistence of stripe-type antiferromagnetic (AFM) and ferromagnetic (FM) spin correlations in both the hole- and electron-doped BaFe 2 As 2 families of iron-pnictide superconductors by a Korringa ratio analysis. Motivated by the NMR work, we investigate the possible existence of FM fluctuations in another iron-pnictide superconducting family, Ca ( Fe 1 - x Co x ) 2 As 2 . We reanalyzed our previously reported data in terms of the Korringa ratio and found clear evidence for the coexistence of stripe-type AFM and FM spin correlations in the electron-doped CaFe 2 As 2 system. These NMR data indicate that FM fluctuations exist in general in iron-pnictide superconducting families and thus must be included to capture the phenomenology of the iron pnictides.

  7. Antiferromagnetic half-metals, gapless half-metals, and spin gapless semiconductors: The D03-type Heusler alloys

    Science.gov (United States)

    Gao, G. Y.; Yao, Kai-Lun

    2013-12-01

    High-spin-polarization materials are desired for the realization of high-performance spintronic devices. We combine recent experimental and theoretical findings to theoretically design several high-spin-polarization materials in binary D03-type Heusler alloys: gapless (zero-gap) half-metallic ferrimagnets of V3Si and V3Ge, half-metallic antiferromagnets of Mn3Al and Mn3Ga, half-metallic ferrimagnets of Mn3Si and Mn3Ge, and a spin gapless semiconductor of Cr3Al. The high spin polarization, zero net magnetic moment, zero energy gap, and slight disorder compared to the ternary and quaternary Heusler alloys make these binary materials promising candidates for spintronic applications. All results are obtained by the electronic structure calculations from first-principles.

  8. Monte Carlo simulations on magnetic behavior of a spin-chain system in triangular lattice doped with antiferromagnetic bonds

    Institute of Scientific and Technical Information of China (English)

    YAO Xiao-yan; LI Peng-lei; DONG Shuai; LIU Jun-ming

    2007-01-01

    A three-dimensional Ising-like model doped with anti-ferromagnetic (AFM) bonds is proposed to investigate the magnetic properties of a doped triangular spin-chain system by using a Monte-Carlo simulation. The simulated results indicate that a steplike magnetization behavior is very sensitive to the concentration of AFM bonds. A low concentration of AFM bonds can suppress the stepwise behavior considerably, in accordance with doping experiments on Ca3Co206. The analysis of spin snapshots demonstrates that the AFM bond doping not only breaks the ferromagnetic ordered linear spin chains along the hexagonal c-axis but also has a great influence upon the spin configuration in the ab-plane.

  9. CP observables with spin-spin correlations in chargino production

    Energy Technology Data Exchange (ETDEWEB)

    Bartl, A. [Faculty of Physics, University of Vienna, Boltzmanngasse 5, A-1090 Wien (Austria); AHEP Group, Institut de Fisica Corpuscular-C.S.I.C., Universitat de Valencia, Edifici Instituts d' Investigacio, Apt. 22085, E-46071 Valencia (Spain); Hohenwarter-Sodek, K. [Faculty of Physics, University of Vienna, Boltzmanngasse 5, A-1090 Wien (Austria); Kernreiter, T. [Faculty of Physics, University of Vienna, Boltzmanngasse 5, A-1090 Wien (Austria)], E-mail: tkern@hephy.oeaw.ac.at; Kittel, O. [Physikalisches Institut der Universitaet Bonn, Nussallee 12, D-53115 Bonn (Germany); Terwort, M. [Institut fuer Experimentalphysik, Universitaet Hamburg, Notkestrasse 85, D-22607 Hamburg (Germany)

    2008-10-11

    We study the CP-violating terms of the spin-spin correlations in chargino production e{sup +}e{sup -}{yields}{chi}-tilde{sub 1}{sup {+-}}{chi}-tilde{sub 2}{sup {+-}}, and their subsequent two-body decays into sneutrinos plus leptons. We propose novel CP-sensitive observables with the help of T-odd products of the spin-spin terms. These terms depend on the polarizations of both charginos, with one polarization perpendicular to the production plane. We identify two classes of CP-sensitive observables; one requires the reconstruction of the production plane, the other not. Our framework is the Minimal Supersymmetric Standard Model with complex parameters.

  10. CP observables with spin-spin correlations in chargino production

    CERN Document Server

    Bartl, Alfred; Kernreiter, T; Kittel, O; Terwort, M

    2008-01-01

    We study the CP-violating terms of the spin-spin correlations in chargino production e+e- -> chi^+/-_1 chi^-/+_2, and their subsequent two-body decays into sneutrinos plus leptons. We propose novel CP-sensitive observables with the help of T-odd products of the spin-spin terms. These terms depend on the polarizations of both charginos, with one polarization perpendicular to the production plane. We identify two classes of CP-sensitive observables; one requires the reconstruction of the production plane, the other not. Our framework is the Minimal Supersymmetric Standard Model with complex parameters. We also calculate the statistical significances to which our CP-sensitive observables can be determined to be non-zero.

  11. Large magnetic cooling power involving frustrated antiferromagnetic spin-glass state in R2NiSi3(R =Gd ,Er )

    Science.gov (United States)

    Pakhira, Santanu; Mazumdar, Chandan; Ranganathan, R.; Giri, S.; Avdeev, Maxim

    2016-09-01

    The ternary intermetallic compounds Gd2NiSi3 and Er2NiSi3 are synthesized in chemically single phase, which are characterized using dc magnetization, ac magnetic susceptibility, heat capacity, and neutron diffraction studies. Neutron diffraction and heat capacity studies confirm that long-range magnetic ordering coexists with the frustrated glassy magnetic components for both compounds. The static and dynamical features of dc magnetization and frequency-dependent ac susceptibility data reveal that Gd2NiSi3 is a canonical spin-glass system, while Er2NiSi3 is a reentrant spin cluster-glass system. The spin freezing temperature merges with the long-range antiferromagnetic ordering temperature at 16.4 K for Gd2NiSi3 . Er2NiSi3 undergoes antiferromagnetic ordering at 5.4 K, which is slightly above the spin freezing temperature at 3 K. The detailed studies of nonequilibrium dynamical behavior, viz., the memory effect and relaxation behavior using different protocols, suggest that both compounds favor the hierarchical model over the droplet model. A large magnetocaloric effect is observed for both compounds. Maximum values of isothermal entropy change (-Δ SM ) and relative cooling power (RCP) are found to be 18.4 J/kg K and 525 J/kg for Gd2NiSi3 and 22.6 J/kg K and 540 J/kg for Er2NiSi3 , respectively, for a change in field from 0 to 70 kOe. The values of RCP are comparable to those of the promising refrigerant materials. A correlation between large RCP and magnetic frustration is discussed for developing new magnetic refrigerant materials.

  12. Off-easy-plane antiferromagnetic spin canting in coupled FePt/NiO bilayer structure with perpendicular exchange bias

    Science.gov (United States)

    Gao, Tenghua; Itokawa, Nobuhide; Wang, Jian; Yu, Youxing; Harumoto, Takashi; Nakamura, Yoshio; Shi, Ji

    2016-08-01

    We report on the investigation of perpendicular exchange bias in FePt (001 ) /NiO (1 ¯1 ¯1 ) orthogonal exchange couple with FePt partially L 10 ordered. From initial magnetization curve measurement and magnetic domain imaging, we find that, for the as-grown bilayer structure, the FePt layer experiences a small-angle magnetization rotation when it is magnetized near to saturation in film normal direction. After field cooling, the bilayer structure shows a significant enhancement of perpendicular magnetic anisotropy, indicating the field mediated coupling between the spins across the FePt/NiO interface. According to Koon's theoretical calculation on the basis of lowest energy ferromagnetic/antiferromagnetic coupling configuration for compensated spins at antiferromagnetic side, we consider slightly slanted Ni spins at the interface off the (1 ¯1 ¯1 ) easy plane can stabilize the spin coupling between FePt and NiO and result in the observed exchange bias in this paper. This consideration was further confirmed by stripe domain width calculation.

  13. LDA+{sigma}({omega}) method for the electronic structure of strongly correlated antiferromagnetic materials: application to La{sub 2}CuO{sub 4}

    Energy Technology Data Exchange (ETDEWEB)

    Perez-Navarro, A.; Costa-Quintana, J.; Lopez-Aguilar, F. [Groupe d' Electromagnetisme, Departament de Fisica, Edifici Cn, Facultat de Ciencies, Universitat Autonoma de Barcelona, 08193 Bellaterra (Barcelona) (Spain)

    2002-09-08

    In this paper we present a method for obtaining the quasiband structure and the renormalized density of quasistates of strongly correlated systems with antiferromagnetic ordering. We calculate the electronic structure of La{sub 2}CuO{sub 4} in order to test this method. The first step required is to calculate the electronic structure from the local density approximation (LDA) in order to obtain the initial non-interacting ground state. The LDA density of states in strongly correlated systems usually presents serious discrepancies with experimental results. As is well known, these discrepancies, fundamentally concerning photoemission, are due to the fact that the dynamic correlation effects are not taken into account within the LDA. In order to include these effects, we obtain a self-energy potential which allows the initial LDA electronic structure to connect with that of the antiferromagnetic ground state arising from a Bogolyubov-like transformation. Within this new ground state, we determine an antiferromagnetic self-energy by means of a spin density wave procedure, and the interacting Green function yields a density of states which is in reasonable agreement with the experimental photoemission result. (Abstract Copyright [2002], Wiley Periodicals, Inc.)

  14. Correlated impurities and intrinsic spin-liquid physics in the kagome material herbertsmithite

    Science.gov (United States)

    Han, Tian-Heng; Norman, M. R.; Wen, J.-J.; Rodriguez-Rivera, Jose A.; Helton, Joel S.; Broholm, Collin; Lee, Young S.

    2016-08-01

    Low energy inelastic neutron scattering on single crystals of the kagome spin-liquid compound ZnCu3(OD) 6Cl2 (herbertsmithite) reveals antiferromagnetic correlations between impurity spins for energy transfers ℏ ω kagome spins. The low energy fluctuations are characterized by diffuse scattering near wave vectors (100) and (00 3/2 ), which is consistent with antiferromagnetic correlations between pairs of nearest-neighbor Cu impurities on adjacent triangular (Zn) interlayers. The corresponding impurity lattice resembles a simple cubic lattice in the dilute limit below the percolation threshold. Such an impurity model can describe prior neutron, NMR, and specific heat data. The low energy neutron data are consistent with the presence of a small spin gap (Δ ˜0.7 meV ) in the kagome layers, similar to that recently observed by NMR. The ability to distinguish the scattering due to Cu impurities from that of the planar kagome Cu spins provides an important avenue for probing intrinsic spin-liquid physics.

  15. Effects of frustration and cyclic exchange on the spin-1/2 Heisenberg antiferromagnet within the self-consistent spin-wave theory

    Science.gov (United States)

    Rutonjski, Milica S.; Pavkov-Hrvojević, Milica V.; Berović, Maja B.

    2016-12-01

    The relevance of the quasi-two-dimensional spin-1/2 frustrated quantum antiferromagnet (AFM) due to its possibility of modeling the high-temperature superconducting parent compounds has resulted in numerous theoretical and experimental studies. This paper presents a detailed research of the influence of the varying exchange interactions on the model magnetic properties within the framework of self-consistent spin-wave theory based on Dyson-Maleev (DM) representation. Beside the nearest neighbor (NN) interaction within the plane, the planar frustration up to the third NNs, cyclic interaction and the interlayer coupling are taken into account. The detailed description of the elementary spin excitations, staggered magnetization, spin-wave velocity renormalization factor and ground state energy is given. The results are compared to the predictions of the linear spin-wave theory and when possible also to the second-order perturbative spin-wave expansion results. Finally, having at our disposal improved experimental results for the in-plane spin-wave dispersion in high-Tc copper oxide La2CuO4, the self-consistent spin-wave theory (SCSWT) is applied to that compound in order to correct earlier obtained set of exchange parameters and high-temperature spin-wave dispersion.

  16. Spin-orbit correlations in the nucleon

    CERN Document Server

    Lorcé, Cédric

    2014-01-01

    We investigate the correlations between the quark spin and orbital angular momentum inside the nucleon. Similarly to the Ji relation, we show that these correlations can be expressed in terms of specific moments of measurable parton distributions. This provides a whole new piece of information about the partonic structure of the nucleon.

  17. Relaxation of a Classical Spin Coupled to a Strongly Correlated Electron System

    Science.gov (United States)

    Sayad, Mohammad; Rausch, Roman; Potthoff, Michael

    2016-09-01

    A classical spin which is antiferromagnetically coupled to a system of strongly correlated conduction electrons is shown to exhibit unconventional real-time dynamics which cannot be described by Gilbert damping. Depending on the strength of the local Coulomb interaction U , the two main electronic dissipation channels, namely transport of excitations via correlated hopping and via excitations of correlation-induced magnetic moments, become active on largely different time scales. We demonstrate that correlations can lead to a strongly suppressed relaxation which so far has been observed in purely electronic systems only and which is governed here by proximity to the divergent magnetic time scale in the infinite-U limit.

  18. Spin-Orbit-Coupled Correlated Metal Phase in Kondo Lattices: An Implementation with Alkaline-Earth Atoms

    Science.gov (United States)

    Isaev, L.; Schachenmayer, J.; Rey, A. M.

    2016-09-01

    We show that an interplay between quantum effects, strong on-site ferromagnetic exchange interaction, and antiferromagnetic correlations in Kondo lattices can give rise to an exotic spin-orbit coupled metallic state in regimes where classical treatments predict a trivial insulating behavior. This phenomenon can be simulated with ultracold alkaline-earth fermionic atoms subject to a laser-induced magnetic field by observing dynamics of spin-charge excitations in quench experiments.

  19. Spin-Orbit-Coupled Correlated Metal Phase in Kondo Lattices: An Implementation with Alkaline-Earth Atoms.

    Science.gov (United States)

    Isaev, L; Schachenmayer, J; Rey, A M

    2016-09-23

    We show that an interplay between quantum effects, strong on-site ferromagnetic exchange interaction, and antiferromagnetic correlations in Kondo lattices can give rise to an exotic spin-orbit coupled metallic state in regimes where classical treatments predict a trivial insulating behavior. This phenomenon can be simulated with ultracold alkaline-earth fermionic atoms subject to a laser-induced magnetic field by observing dynamics of spin-charge excitations in quench experiments.

  20. Observation of spatial charge and spin correlations in the 2D Fermi-Hubbard model.

    Science.gov (United States)

    Cheuk, Lawrence W; Nichols, Matthew A; Lawrence, Katherine R; Okan, Melih; Zhang, Hao; Khatami, Ehsan; Trivedi, Nandini; Paiva, Thereza; Rigol, Marcos; Zwierlein, Martin W

    2016-09-16

    Strong electron correlations lie at the origin of high-temperature superconductivity. Its essence is believed to be captured by the Fermi-Hubbard model of repulsively interacting fermions on a lattice. Here we report on the site-resolved observation of charge and spin correlations in the two-dimensional (2D) Fermi-Hubbard model realized with ultracold atoms. Antiferromagnetic spin correlations are maximal at half-filling and weaken monotonically upon doping. At large doping, nearest-neighbor correlations between singly charged sites are negative, revealing the formation of a correlation hole, the suppressed probability of finding two fermions near each other. As the doping is reduced, the correlations become positive, signaling strong bunching of doublons and holes, in agreement with numerical calculations. The dynamics of the doublon-hole correlations should play an important role for transport in the Fermi-Hubbard model.

  1. Topological Phases of Spin-1/2 Ferromagnetic-Antiferromagnetic Alternating Heisenberg Chains with Alternating Next-Nearest-Neighbour Interaction

    Science.gov (United States)

    Hida, Kazuo

    2016-12-01

    A series of symmetry-protected topological (SPT) and trivial spin-gap phases in the spin-1/2 ferromagnetic-antiferromagnetic alternating Heisenberg chain with alternating next-nearest-neighbour interaction are investigated using two kinds of entanglement spectra defined by different divisions of the whole chain. In case one of the next-nearest-neighbor interactions vanishes, the model reduces to the Δ-chain in which a series of spin-gap phases are found, as shown in J. Phys. Soc. Jpn. 77, 044707 (2008). From the degeneracy of the entanglement spectra, these phases are identified as the SPT and trivial phases. It is found that the ground-state phase boundaries are insensitive to the strength of the alternation in the next-nearest-neighbor interaction. These results are consistent with the analysis based on the nonlinear σ model and exact solution on the ferromagnetic-nonmagnetic phase boundary.

  2. Neutron scattering studies of two-dimensional antiferromagnetic spin fluctuations in insulating and superconducting S = ½ systems

    DEFF Research Database (Denmark)

    Christensen, Niels Bech

    polarized multimagnon excitations is discovered at energies above the single-magnon branch. At low energies, the findings are well described bylinear spin wave theory. At high energies, linear spin wave theory fails and instead the data are very well accounted for by state-of-the-art Quantum Monte Carlo......Time-of-flight and polarized triple axis neutron scattering is used to probe the spin excitations of Cu(DCOO)_2_·_4D_2O and La_2_-_xSr_xCuO_4. The first part of the thesis contains an investigation of the excitation spectrum of the square lattice S = 1/2Heisenberg antiferromagnet Cu(DCOO)_2_·_4D_2O...

  3. The spin-half XXZ antiferromagnet on the square lattice revisited: A high-order coupled cluster treatment

    Science.gov (United States)

    Bishop, R. F.; Li, P. H. Y.; Zinke, R.; Darradi, R.; Richter, J.; Farnell, D. J. J.; Schulenburg, J.

    2017-04-01

    We use the coupled cluster method (CCM) to study the ground-state properties and lowest-lying triplet excited state of the spin-half XXZ antiferromagnet on the square lattice. The CCM is applied to it to high orders of approximation by using an efficient computer code that has been written by us and which has been implemented to run on massively parallelized computer platforms. We are able therefore to present precise data for the basic quantities of this model over a wide range of values for the anisotropy parameter Δ in the range - 1 ≤ Δ 1) regimes, where Δ → ∞ represents the Ising limit. We present results for the ground-state energy, the sublattice magnetization, the zero-field transverse magnetic susceptibility, the spin stiffness, and the triplet spin gap. Our results provide a useful yardstick against which other approximate methods and/or experimental studies of relevant antiferromagnetic square-lattice compounds may now compare their own results. We also focus particular attention on the behaviour of these parameters for the easy-axis system in the vicinity of the isotropic Heisenberg point (Δ = 1) , where the model undergoes a phase transition from a gapped state (for Δ > 1) to a gapless state (for Δ ≤ 1), and compare our results there with those from spin-wave theory (SWT). Interestingly, the nature of the criticality at Δ = 1 for the present model with spins of spin quantum number s =1/2 that is revealed by our CCM results seems to differ qualitatively from that predicted by SWT, which becomes exact only for its near-classical large-s counterpart.

  4. Relaxation of antiferromagnetic order in spin-1/2 chains following a quantum quench.

    Science.gov (United States)

    Barmettler, Peter; Punk, Matthias; Gritsev, Vladimir; Demler, Eugene; Altman, Ehud

    2009-04-03

    We study the unitary time evolution of antiferromagnetic order in anisotropic Heisenberg chains that are initially prepared in a pure quantum state far from equilibrium. Our analysis indicates that the antiferromagnetic order imprinted in the initial state vanishes exponentially. Depending on the anisotropy parameter, oscillatory or nonoscillatory relaxation dynamics is observed. Furthermore, the corresponding relaxation time exhibits a minimum at the critical point, in contrast to the usual notion of critical slowing down, from which a maximum is expected.

  5. Spin Dynamics and Critical Fluctuations in a Two-Dimensional Random Antiferromagnet

    DEFF Research Database (Denmark)

    Als-Nielsen, Jens Aage; Birgeneau, R. J.; Guggenheim, H. J.

    1975-01-01

    A comprehensive elastic- and inelastic-neutron-scattering study of the binary mixed antiferromagnet Rb2Mn0.5Ni0.5F4 has been carried out. The pure materials, Rb2MnF4 and Rb2NiF4 are [2d] near-Heisenberg antiferromagnets of the K2NiF4 type. Elastic-scattering experiments demonstrate that the Mn...

  6. Fullerene antiferromagnetic reconstructed spinterface subsurface layer dominates multi-orbitals spin-splitting and large magnetic moment in C60

    CERN Document Server

    Shao, Yangfan; Pan, Hui; Shi, Xingqiang

    2016-01-01

    The interfaces between organic molecules and metal surfaces with layered antiferromagnetic order have gained increasing interests in the field of antiferromagnetic spintronics. The C60 layered AFM spinterfaces have been studied for C60 bonded only to the outermost ferromagnetic layer. Using density functional theory calculations, here we demonstrate that C60 adsorption can reconstruct the layered AFM Cr(001) surface so that C60 bonds to the top two Cr layers with opposite spin direction. Surface reconstruction drastically changes C60 s spintronic properties 1 the spin-split p-d hybridization involve multi-orbitals of C60 and metal double layers, 2 the subsurface layer dominates the C60 spin properties, and 3) reconstruction induces a large magnetic moment in C60 of 0.58 B, which is a synergetic effect of the top two layers as a result of a magnetic direct-exchange interaction. Understanding these complex spinterfaces phenomena is a crucial step for their device applications. The surface reconstruction can be ...

  7. Magnetic properties of the S = 1/2 antiferromagnetic spin-chain α - Cu2V2O7

    Science.gov (United States)

    Gitgeatpong, Ganatee; Zhao, Yang; Avdeev, Maxim; Piltz, Ross; Sato, Taku; Matan, Kittiwit

    2015-03-01

    Magnetic properties of the S = 1 / 2 antiferromagnetic spin-chain, α - Cu2V2O7, have been studied using magnetization and neutron scattering measurements on powder and single-crystal samples. Magnetic susceptibility reveals a Curie-Weiss temperature of Θ = -73.2(9) K with a magnetic phase transition at TN = 33 K while the Bonner-Fisher fit to the magnetic susceptibility for T >TN with magnetic field perpendicular to the crystallographic a - axis yields the intra-chain coupling of |J|/k = 46.0(2) K. Small ferromagnetism below TN is due to spin-canting caused by Dzyaloshinskii-Moriya interactions. Analysis of the neutron diffraction data reveals that the Cu2+ spins are coupled antiferromagnetically along zigzag chains, which run alternately along [011] and [01-1] directions. The ordered moment of 0.925(3) μB is predominantly along the a - axis. Our recent inelastic neutron scattering, which reveals atypical magnetic excitations centered at commensurate wave vectors (0, +/-0.25, 0) around the magnetic zone center, will also be discussed.

  8. Doping dependence of spin excitations and its correlations with high-temperature superconductivity in iron pnictides.

    Science.gov (United States)

    Wang, Meng; Zhang, Chenglin; Lu, Xingye; Tan, Guotai; Luo, Huiqian; Song, Yu; Wang, Miaoyin; Zhang, Xiaotian; Goremychkin, E A; Perring, T G; Maier, T A; Yin, Zhiping; Haule, Kristjan; Kotliar, Gabriel; Dai, Pengcheng

    2013-01-01

    High-temperature superconductivity in iron pnictides occurs when electrons and holes are doped into their antiferromagnetic parent compounds. Since spin excitations may be responsible for electron pairing and superconductivity, it is important to determine their electron/hole-doping evolution and connection with superconductivity. Here we use inelastic neutron scattering to show that while electron doping to the antiferromagnetic BaFe₂As₂ parent compound modifies the low-energy spin excitations and their correlation with superconductivity (100 meV), hole-doping suppresses the high-energy spin excitations and shifts the magnetic spectral weight to low-energies. In addition, our absolute spin susceptibility measurements for the optimally hole-doped iron pnictide reveal that the change in magnetic exchange energy below and above T(c) can account for the superconducting condensation energy. These results suggest that high-T(c) superconductivity in iron pnictides is associated with both the presence of high-energy spin excitations and a coupling between low-energy spin excitations and itinerant electrons.

  9. Electron spin resonance study of the single-ion anisotropy in the pyrochlore antiferromagnet Gd2Sn2O7

    Science.gov (United States)

    Glazkov, V. N.; Smirnov, A. I.; Sanchez, J. P.; Forget, A.; Colson, D.; Bonville, P.

    2006-02-01

    Single-ion anisotropy is of importance for the magnetic ordering of the frustrated pyrochlore antiferromagnets Gd2Ti2O7 and Gd2Sn2O7. The anisotropy parameters for Gd2Sn2O7 were measured using the electron spin resonance technique. The anisotropy was found to be of the easy plane type, with the main constant D = 140 mK. This value is 35% smaller than the value of the corresponding anisotropy constant of the related compound Gd2Ti2O7.

  10. The magnetic properties of a quasi-two-dimensional spin 1 easy axis Heisenberg antiferromagnet with competing interactions

    Energy Technology Data Exchange (ETDEWEB)

    Sousa, Griffith Mendonça A., E-mail: griffith_mas@hotmail.com; Pires, A.S.T.

    2014-03-15

    The Neel and collinear ordered phases of the two-dimensional S=1 antiferromagnet with next and next near neighbor exchange interactions and easy axis single ion anisotropy, on the square lattice, are studied at low temperature using a Modified Spin Wave Theory. We calculate the low-temperature quantities as a function of the temperature, frustration and anisotropy. We calculate also the phase diagram at T=0. We found a disordered phase separating the Neel and collinear phases. - Highlights: • The phase diagrams in zero temperature. • The critical temperature was studied as a function of frustration and D. • The sublattice magnetizations and the gap were studied.

  11. A new correlator in quantum spin chains

    Energy Technology Data Exchange (ETDEWEB)

    Keating, J P; Mezzadri, F; Novaes, M [School of Mathematics, University of Bristol, Bristol BS8 1TW (United Kingdom)

    2006-06-16

    We propose a new correlator in one-dimensional quantum spin chains, the s-emptiness formation probability (s-EFP). This is a generalization of the emptiness formation probability (EFP), which is the probability that the first n spins of the chain are all aligned downwards. In the s-EFP we let the spins in question be separated by s sites. The usual EFP corresponds to the special case when s = 1. Taking s > 1 allows us to quantify non-local correlations. We express the s-EFP for the anisotropic XY model in a transverse magnetic field, a system with both critical and non-critical regimes, in terms of a Toeplitz determinant. For the isotropic XY model we find that the magnetic field induces an interesting length scale. (letter to the editor)

  12. Critical spin dynamics of the 2D quantum Heisenberg antiferromagnets Sr2CuO2Cl2 and Sr2Cu3O4Cl2.

    Science.gov (United States)

    Kim, Y J; Birgeneau, R J; Chou, F C; Erwin, R W; Kastner, M A

    2001-04-02

    We report a neutron scattering study of the long-wavelength dynamic spin correlations in the model two-dimensional S = 1/2 square lattice Heisenberg antiferromagnets Sr2CuO2Cl2 and Sr2Cu3O4Cl2. The characteristic energy scale, omega(0)(T/J), is determined by measuring the quasielastic peak width in the paramagnetic phase over a wide range of temperature ( 0.2 less similarT/J less similar0.7). The obtained values for omega(0)(T/J) agree quantitatively between the two compounds and also with values deduced from quantum Monte Carlo simulations. The combined data show scaling behavior, omega approximately xi(-z), over the entire temperature range with z = 1.0(1), in agreement with dynamic scaling theory.

  13. Plaquette-triplon analysis of magnetic disorder and order in a trimerized spin-1 kagome Heisenberg antiferromagnet

    Science.gov (United States)

    Ghosh, Pratyay; Verma, Akhilesh Kumar; Kumar, Brijesh

    2016-01-01

    A spin-1 Heisenberg model on trimerized kagome lattice is studied by doing a low-energy bosonic theory in terms of plaquette triplons defined on its triangular unit cells. The model considered has an intratriangle antiferromagnetic exchange interaction J (set to 1) and two intertriangle couplings J'>0 (nearest neighbor) and J″ (next nearest neighbor; of both signs). The triplon analysis performed on this model investigates the stability of the trimerized singlet ground state (which is exact in the absence of intertriangle couplings) in the J'-J″ plane. It gives a quantum phase diagram that has two gapless antiferromagnetically ordered phases separated by the spin-gapped trimerized singlet phase. The trimerized singlet ground state is found to be stable on J″=0 line (the nearest-neighbor case), and on both sides of it for J″≠0 , in an extended region bounded by the critical lines of transition to the gapless antiferromagnetic phases. The gapless phase in the negative J″ region has a coplanar 120∘ antiferromagnetic order with √{3 }×√{3 } structure. In this phase, all the magnetic moments are of equal length, and the angle between any two of them on a triangle is exactly 120∘. The magnetic lattice in this case has a unit cell consisting of three triangles. The other gapless phase, in the positive J″ region, is found to exhibit a different coplanar antiferromagnetic order with ordering wave vector q =(0 ,0 ) . Here, two magnetic moments in a triangle are of the same magnitude, but shorter than the third. While the angle between two short moments is 120∘-2 δ , it is 120∘+δ between a short and the long one. Only when J″=J' , their magnitudes become equal and the relative angles 120∘. The magnetic lattice in this q =(0 ,0 ) phase has the translational symmetry of the kagome lattice with triangular unit cells of reduced (isosceles) symmetry. This reduction in the point-group symmetry is found to show up as a difference in the intensities of

  14. Low temperature magnetic properties and spin dynamics in single crystals of Cr{sub 8}Zn antiferromagnetic molecular rings

    Energy Technology Data Exchange (ETDEWEB)

    Adelnia, Fatemeh [Dipartimento di Fisica, Università degli Studi di Milano and INSTM, I-20133 Milano (Italy); Dipartimento di Fisica, Università degli Studi di Pavia and INSTM, I-27100 Pavia (Italy); Chiesa, Alessandro; Bordignon, Sara; Carretta, Stefano [Dipartimento di Fisica e Scienze della Terra, Università degli Studi di Parma, I-43124 Parma (Italy); Ghirri, Alberto; Candini, Andrea [CNR Institute Nanosciences S3, I- 41125 Modena (Italy); Cervetti, Christian [Dipartimento di Scienze Fisiche, Informatiche, Matematiche, Università di Modena e Reggio Emilia, I-41125 Modena (Italy); Evangelisti, Marco [CNR Institute Nanosciences S3, I- 41125 Modena (Italy); Dipartimento di Scienze Fisiche, Informatiche, Matematiche, Università di Modena e Reggio Emilia, I-41125 Modena (Italy); Instituto de Ciencia de Materiales de Aragón and Departamento de Física de la Materia Condensada, CSIC-Universidad de Zaragoza, 50009 Zaragoza (Spain); Affronte, Marco [CNR Institute Nanosciences S3, I- 41125 Modena (Italy); Dipartimento di Scienze Fisiche, Informatiche, Matematiche, Università di Modena e Reggio Emilia, I-41125 Modena (Italy); Sheikin, Ilya [Grenoble High Magnetic Field Laboratory, CNRS-LNCMI, 25, B.P. 166, 38042 Grenoble Cedex 9 (France); Winpenny, Richard; Timco, Grigore [The Lewis Magnetism Laboratory, The University of Manchester, M13 9PL Manchester (United Kingdom); Borsa, Ferdinando [Dipartimento di Fisica, Università degli Studi di Pavia and INSTM, I-27100 Pavia (Italy); and others

    2015-12-28

    A detailed experimental investigation of the effects giving rise to the magnetic energy level structure in the vicinity of the level crossing (LC) at low temperature is reported for the open antiferromagnetic molecular ring Cr{sub 8}Zn. The study is conducted by means of thermodynamic techniques (torque magnetometry, magnetization and specific heat measurements) and microscopic techniques (nuclear magnetic resonance line width, nuclear spin lattice, and spin-spin relaxation measurements). The experimental results are shown to be in excellent agreement with theoretical calculations based on a minimal spin model Hamiltonian, which includes a Dzyaloshinskii-Moriya interaction. The first ground state level crossing at μ{sub 0}H{sub c1} = 2.15 T is found to be an almost true LC while the second LC at μ{sub 0}H{sub c2} = 6.95 T has an anti-crossing gap of Δ{sub 12} = 0.19 K. In addition, both NMR and specific heat measurements show the presence of a level anti-crossing between excited states at μ{sub 0}H = 4.5 T as predicted by the theory. In all cases, the fit of the experimental data is improved by introducing a distribution of the isotropic exchange couplings (J), i.e., using a J strain model. The peaks at the first and second LCs in the nuclear spin-lattice relaxation rate are dominated by inelastic scattering and a value of Γ ∼ 10{sup 10} rad/s is inferred for the life time broadening of the excited state of the open ring, due to spin phonon interaction. A loss of NMR signal (wipe-out effect) is observed for the first time at LC and is explained by the enhancement of the spin-spin relaxation rate due to the inelastic scattering.

  15. Antiferromagnetic spin cantings as a driving force of ferroelectricity in multiferroic Cu2OSeO3

    Science.gov (United States)

    Chizhikov, Viacheslav A.; Dmitrienko, Vladimir E.

    2017-04-01

    Ferroelectric properties of cubic chiral magnet Cu2OSeO3 can emerge due to the spin noncollinearity induced by antiferromagnetic cantings. The cantings are the result of the Dzyaloshinskii–Moriya interaction and in many ways similar to the ferromagnetic cantings in weak ferromagnets. An expression for the local electric polarization is derived, including terms with gradients of magnetization \\mathbf{M}≤ft(\\mathbf{r}\\right) . When averaged over the crystal the electric polarization has a non-vanishing part associated with the anisotropy of the crystal point group 23. In the framework of the microscopic theory, it is shown that both scalar and vector products of spins, ≤ft({{\\mathbf{s}}1}\\cdot {{\\mathbf{s}}2}\\right) and ≤ft[{{\\mathbf{s}}1}× {{\\mathbf{s}}2}\\right] , can give contributions of the same order of magnitude into the electric polarization.

  16. Magnetism and thermodynamics of the anisotropic frustrated spin-1 Heisenberg antiferromagnet on a body-centered cubic lattice

    Science.gov (United States)

    Mi, Bin-Zhou

    2017-02-01

    The magnetic and thermodynamic properties of anisotropic frustrated spin-1 Heisenberg antiferromagnet on a body-centered cubic lattice for Néel phase (the region of weak frustration) are systematically investigated by use of the double-time Green's function method within the random phase approximation and the Anderson and Callen's decoupling. The zero-temperature sublattice magnetization and Néel temperature increase with spin anisotropy strength and single-ion anisotropy strength, and decrease with frustration strength. This indicates that quantum fluctuation is suppressed by spin anisotropy and single-ion anisotropy, by contrast, is strengthened by frustration. It is possible to tune the quantum fluctuations by the competition of anisotropy strength and frustration strength to change the ground state properties of magnetic materials. Although we find that both the spin anisotropy and the single-ion anisotropy suppress the quantum fluctuations, but their respective effects on the thermodynamic quantities, especially the internal energy and free energy, are different at zero temperature and finite temperature. Furthermore, when these two kinds of anisotropic coexist, the effect of the spin anisotropy on the sublattice magnetization and internal energy is larger than that of the single-ion anisotropy.

  17. Electronic properties of antiferromagnetic UBi2 metal by exact exchange for correlated electrons method

    Directory of Open Access Journals (Sweden)

    E Ghasemikhah

    2012-03-01

    Full Text Available This study investigated the electronic properties of antiferromagnetic UBi2 metal by using ab initio calculations based on the density functional theory (DFT, employing the augmented plane waves plus local orbital method. We used the exact exchange for correlated electrons (EECE method to calculate the exchange-correlation energy under a variety of hybrid functionals. Electric field gradients (EFGs at the uranium site in UBi2 compound were calculated and compared with the experiment. The EFGs were predicted experimentally at the U site to be very small in this compound. The EFG calculated by the EECE functional are in agreement with the experiment. The densities of states (DOSs show that 5f U orbital is hybrided with the other orbitals. The plotted Fermi surfaces show that there are two kinds of charges on Fermi surface of this compound.

  18. Disappearance of antiferromagnetic spin excitations in overdoped La2-xSrxCuO4.

    Science.gov (United States)

    Wakimoto, S; Yamada, K; Tranquada, J M; Frost, C D; Birgeneau, R J; Zhang, H

    2007-06-15

    Magnetic excitations for energies up to approximately 100 meV are studied for overdoped La(2-x)Sr(x)CuO(4) with x=0.25 and 0.30, using time-of-flight neutron spectroscopy. Comparison of spectra integrated over the width of an antiferromagnetic Brillouin zone demonstrates that the magnetic scattering at intermediate energies, 20 antiferromagnetic bubbles.

  19. Neutron scattering studies of two-dimensional antiferromagnetic spin fluctuations in insulating and superconducting S = 1/2 systems

    Energy Technology Data Exchange (ETDEWEB)

    Bech Christensen, N

    2005-01-01

    Time-of-flight and polarized triple axis neutron scattering is used to probe the spin excitations of Cu(DCOO){sub 2}x4D{sub 2}O and La{sub 2-x}Sr{sub x}CuO{sub 4}. The first part of the thesis contains an investigation of the excitation spectrum of the square lattice S = 1/2 Heisenberg antiferromagnet Cu(DCOO){sub 2}4D{sub 2}O. Along the antiferromagnetic zone boundary a pronounced intensity variation is found for the dominant single-magnon excitations. This variation tracks an already known zone boundary dispersion. Using polarization analysis to separate the components of the excitation spectrum, a continuum of longitudinally polarized multimagnon excitations is discovered at energies above the single-magnon branch. At low energies, the findings are well described by linear spin wave theory. At high energies, linear spin wave theory fails and instead the data are very well accounted for by state-of-the-art Quantum Monte Carlo computations. In the second part of the thesis, the spin excitation spectra of the high temperature superconductors La{sub 1.90}Sr{sub 0.10}CuO{sub 4} and La{sub 1.84}Sr{sub 0.16}Cu characterized. The main discovery is that the excitations are dispersive at both doping levels. The dispersion strongly resembles that seen in other high-T{sub c} superconductors. The presence of dispersive excitations does not require superconductivity to exist. For La{sub 1.84}Sr{sub 0.16}CuO{sub 4}, but not for La{sub 1.90}Sr{sub 0.10}CuO{sub 4}, the onset superconductivity gives rise to a spectral weight shift which displays qualitative and quantitative similarities to the resonance mode observed in other high-T{sub c} superconductors. (au)

  20. Thermodynamic and Neutron Scattering Study of the Spin-1/2 Kagome Antiferromagnet ZnCu3(OH)6Cl2: A Quantum Spin Liquid System

    Science.gov (United States)

    Han, Tianheng

    New physics, such as a quantum spin liquid, can emerge in systems where quantum fluctuations are enhanced due to reduced dimensionality and strong frustration . The realization of a quantum spin liquid in two-dimensions would represent a new state of matter. It is believed that spin liquid physics plays a role in the phenomenon of high-Tc superconductivity, and the topological properties of the spin liquid state may have applications in the field of quantum information. The Zn-paratacamite family, ZnxCu4-- x(OH)6Cl2 for x > 0.33, is an ideal system to look for such an exotic state in the form of antiferromagnetic Cu 2 + kagome planes. The x = 1 end member, named herbertsmithite, has shown promising spin liquid properties from prior studies on powder samples. Here we show a new synthesis by which high-quality centimeter-sized single crystals of Znparatacamite have been produced for the first time. Neutron and synchrotron xray diffraction experiments indicate no structural transition down to T = 2 K. The magnetic susceptibility both perpendicular and parallel to the kagome plane has been measured for the x = 1 sample. A small, temperature-dependent anisotropy has been observed, where chi z / chip > 1 at high temperatures and chiz / chip fingerprint of the quantum spin liquid state in herbertsmithite. (Copies available exclusively from MIT Libraries, libraries.mit.edu/docs - docs mit.edu)

  1. Quantum Monte Carlo simulation of antiferromagnetic spin ladder (C5H12N)2CuBr4

    Science.gov (United States)

    Freitas, Augusto S.

    2016-07-01

    In this paper I present a Quantum Monte Carlo (QMC) study of the magnetic properties of an antiferromagnetic spin ladder (C5H12N)2CuBr4. This compound is the prototype of the Heisenberg model for a two leg spin ladder in the presence of an external magnetic field. The susceptibility phase diagram has a rounded peak in the vicinity of T=7.4 K, obeys Troyer's law for low temperatures, and Curie's law for high temperatures. I also study the susceptibility diagram in low temperatures and I found the spin gap Δ=9.26 K, in good concordance with the experimental value, 9.5 K. In high field, I present a diagram of magnetization as a function of temperature. In the vicinity of a critical field, Hci, the magnetization scales with T1/2 and this result was found also in the QMC simulation. In all the results, there is a very good concordance with the experimental data. I also show in this paper that the spin gap is null and the susceptibility is proportional to T for low temperatures when relatively high values of the ladders' coupling is taken in account.

  2. Anomalous Hall effect and spin-orbit torques in MnGa/IrMn films: Modification from strong spin Hall effect of the antiferromagnet

    Science.gov (United States)

    Meng, K. K.; Miao, J.; Xu, X. G.; Wu, Y.; Zhao, X. P.; Zhao, J. H.; Jiang, Y.

    2016-12-01

    We report systematic measurements of anomalous Hall effect (AHE) and spin-orbit torques (SOTs) in MnGa/IrMn films, in which a single L 10-MnGa epitaxial layer reveals obvious orbital two-channel Kondo (2CK) effect. As increasing the thickness of the antiferromagnet IrMn, the strong spin Hall effect (SHE) has gradually suppressed the orbital 2CK effect and modified the AHE of MnGa. A scaling involving multiple competing scattering mechanisms has been used to distinguish different contributions to the modified AHE. Finally, the sizeable SOT in the MnGa/IrMn films induced by the strong SHE of IrMn have been investigated. The IrMn layer also supplies an in-plane exchange bias field and enables nearly field-free magnetization reversal.

  3. The anisotropic quantum spin-1/2 Heisenberg antiferromagnet in the presence of a longitudinal field on a bcc lattice

    Energy Technology Data Exchange (ETDEWEB)

    Neto, Minos A., E-mail: minos@pq.cnpq.br [Departamento de Fisica, Universidade Federal do Amazonas, 3000, Japiim, Manaus, 69077-000 AM (Brazil); Roberto Viana, J., E-mail: vianafisica@bol.com.br [Departamento de Fisica, Universidade Federal do Amazonas, 3000, Japiim, Manaus, 69077-000 AM (Brazil); Ricardo de Sousa, J., E-mail: jsousa@edu.ufam.br [Departamento de Fisica, Universidade Federal do Amazonas, 3000, Japiim, Manaus, 69077-000 AM (Brazil); National Institute of Science and Technology for Complex Systems, 3000, Japiim, Manaus, 69077-000 AM (Brazil)

    2012-08-15

    In this work we study the critical behavior of the quantum spin-1/2 anisotropic Heisenberg antiferromagnet in the presence of a longitudinal field on a body centered cubic (bcc) lattice as a function of temperature, anisotropy parameter ({Delta}) and magnetic field (H), where {Delta}=0 and 1 correspond the isotropic Heisenberg and Ising models, respectively. We use the framework of the differential operator technique in the effective-field theory with finite cluster of N=4 spins (EFT-4). The staggered m{sub s}=(m{sub A}-m{sub B})/2 and total m=(m{sub A}+m{sub B})/2 magnetizations are numerically calculated, where in the limit of m{sub s}{yields}0 the critical line T{sub N}(H,{Delta}) is obtained. The phase diagram in the T-H plane is discussed as a function of the parameter {Delta} for all values of H Element-Of [0,H{sub c}({Delta})], where H{sub c}({Delta}) correspond the critical field (T{sub N}=0). Special focus is given in the low temperature region, where a reentrant behavior is observed around of H=H{sub c}({Delta}){>=}H{sub c}({Delta}=1)=8J in the Ising limit, results in accordance with Monte Carlo simulation, and also was observed for all values of {Delta} Element-Of [0,1]. This reentrant behavior increases with increase of the anisotropy parameter {Delta}. In the limit of low field, our results for the Heisenberg limit are compared with series expansion values. - Highlights: Black-Right-Pointing-Pointer In the lat decade there has been a great interest in the physics of the quantum phase transition in spins system. Black-Right-Pointing-Pointer Effective-field theory in cluster with N=4 spins is generalized to treat the quantum spin-1/2 Heisenberg model. Black-Right-Pointing-Pointer We have obtained phase diagram at finite temperature for the quantum spin-1/2 antiferromagnet Heisenberg model as a bcc lattice.

  4. Magnetic correlations in the 2D S=5/2 honeycomb antiferromagnet MnPS3

    DEFF Research Database (Denmark)

    Rønnow, H.M.; Wildes, A.R.; Bramwell, S.T.

    2000-01-01

    MnPS3 is a quasi-2D S = 5/2 antiferromagnet on a honeycomb lattice. Using an energy integrating neutron scattering technique, we have measured the structure factor S(k) of the instantaneous magnetic fluctuations. The temperature dependence of the correlation length xi follows the Kosterlitz...

  5. Characterisation of spin-waves in copper(II) deuteroformate tetradeuterate: A square ¤S¤=1/2 Heisenberg antiferromagnet

    DEFF Research Database (Denmark)

    Clarke, S.J.; Harrison, A.; Mason, T.E.;

    1999-01-01

    Copper(II) formate tetrahydrate (CFTH) is a model square S = 1/2 Heisenberg antiferromagnet with T-N = 16.54 +/- 0.05 K. The dispersion of spin-waves in the magnetic layers of a fully deuterated sample of this material has been mapped at 4.3 K by inelastic neutron scattering from the zone centre...

  6. Quantum features in the spin dynamics of S=1/2 and 1 Heisenberg antiferromagnets in spite of long-range ordered phases

    DEFF Research Database (Denmark)

    Enderle, M.; Kiefer, K.; Klopperpieper, A.;

    2000-01-01

    Uniform S = 1 and 1/2 Heisenberg antiferromagnetic chains have a quantum singlet ground state which is an eigenstate of the total spin with S(tot) = 0. However, the 'internal' order of these ground states is quite different, and is reflected in gapless excitations in the S = 1/2 state, while the S...

  7. Erratum : Critical Properties of Spin-1 Antiferromagnetic Heisenberg Chains with Bond Alternation and Uniaxial Single-Ion-Type Anisotropy (vol 69, pg 237, 2000)

    OpenAIRE

    飛田, 和男

    2008-01-01

    Original Paper :Critical Properties of Spin-1 Antiferromagnetic Heisenberg Chains with Bond Alternation and Uniaxial Single-Ion-Type AnisotropyWei Chen, Kazuo Hida and Bryan Clifford Sanctuary Journal of the Physical Society of Japan 69 (2000) pp.237-241

  8. Spin frustration and magnetic ordering in triangular lattice antiferromagnet Ca3CoNb2O9

    Science.gov (United States)

    Dai, Jia; Zhou, Ping; Wang, Peng-Shuai; Pang, Fei; Munsie, Tim J.; Luke, Graeme M.; Zhang, Jin-Shan; Yu, Wei-Qiang

    2015-12-01

    We synthesized a quasi-two-dimensional distorted triangular lattice antiferromagnet Ca3CoNb2O9, in which the effective spin of Co2+ is 1/2 at low temperatures, whose magnetic properties were studied by dc susceptibility and magnetization techniques. The x-ray diffraction confirms the quality of our powder samples. The large Weiss constant θCW˜ -55 K and the low Neel temperature TN˜ 1.45 K give a frustration factor f = | θCW/TN | ≈ 38, suggesting that Ca3CoNb2O9 resides in strong frustration regime. Slightly below TN, deviation between the susceptibility data under zero-field cooling (ZFC) and field cooling (FC) is observed. A new magnetic state with 1/3 of the saturate magnetization Ms is suggested in the magnetization curve at 0.46 K. Our study indicates that Ca3CoNb2O9 is an interesting material to investigate magnetism in triangular lattice antiferromagnets with weak anisotropy. Project supported by the National Natural Science Foundation of China (Grant Nos. 11374364 and 11222433), the National Basic Research Program of China (Grant No. 2011CBA00112). Research at McMaster University supported by the Natural Sciences and Engineering Research Council. Work at North China Electric Power University supported by the Scientific Research Foundation for the Returned Overseas Chinese Scholars, State Education Ministry.

  9. Charge stripes and spin correlations in copper-oxide superconductors

    Science.gov (United States)

    Tranquada, J. M.

    1997-08-01

    Recent neutron diffraction studies have yielded evidence that, in a particular cuprate family, holes doped into the CuO 2 planes segregate into stripes that separate antiferromagnetic domains. Here it is shown that such a picture provides a quantitatively consistent interpretation of the spin fluctuations measured by neutron diffraction in La 1.85Sr 0.15CuO 4 and YBa 2Cu 3O 6+ x.

  10. Charge stripes and spin correlations in copper-oxide superconductors

    OpenAIRE

    Tranquada, J. M.

    1997-01-01

    Recent neutron diffraction studies have yielded evidence that, in a particular cuprate family, holes doped into the CuO(2) planes segregate into stripes that separate antiferromagnetic domains. Here it is shown that such a picture provides a quantitatively consistent interpretation of the spin fluctuations measured by neutron scattering in La(1.85)Sr(0.15)CuO(4) and YBa(2)Cu(3)O(6+x).

  11. Spin-glass, antiferromagnetism and Kondo behavior in Ce2Au1-CoSi3 alloys

    Indian Academy of Sciences (India)

    Subham Majumdar; E V Sampathkumaran; St Berger; M Della Mea; H Michor; E Bauer; M Brando; J Hemberger; A Loidl

    2002-05-01

    Recently, the solid solution Ce2Au1-CoSi3 has been shown to exhibit many magnetic anomalies associated with the competition between magnetic ordering and the Kondo effect. Here we report high pressure electrical resistivity of Ce2AuSi3, ac susceptibility () and magnetoresistance of various alloys of this solid solution in order to gain better knowledge of the magnetism of these alloys. High pressure resistivity behavior is consistent with the proposal that Ce2AuSi3 lies at the left-hand side of the maximum in Doniach’s magnetic phase diagram. The ac data reveal that there are in fact two magnetic transitions, one at 2 K and the other at 3 K for this compound, both of which are spin-glass-like. However, as the Co concentration is increased, antiferromagnetism is stabilized for intermediate compositions before attaining non-magnetism for the Co end member.

  12. Geometric frustration effects in the spin-1 antiferromagnetic Ising model on the kagome-like recursive lattice: exact results

    Science.gov (United States)

    Jurčišinová, E.; Jurčišin, M.

    2016-09-01

    The antiferromagnetic spin-1 Ising model is studied on the Husimi lattice constructed from elementary triangles with coordination number z  =  4. It is found that the model has a unique solution for arbitrary values of the magnetic field as well as for all temperatures. A detailed analysis of the magnetization is performed and it is shown that in addition to the standard plateau-like ground states, the model also contains well-defined single-point ground states related to definite values of the magnetic field. Exact values of the residual entropies for all ground states are found. The properties of the susceptibility and the specific heat of the model are also discussed. The existence of the Schottky-type behavior of the specific heat and the strong magnetocaloric effect for low enough temperatures and for the external magnetic field close to the values at which the single-point ground states exist are identified.

  13. Quantum phase transition, universality, and scaling behaviors in the spin-1/2 Heisenberg model with ferromagnetic and antiferromagnetic competing interactions on a honeycomb lattice

    Science.gov (United States)

    Huang, Yi-Zhen; Xi, Bin; Chen, Xi; Li, Wei; Wang, Zheng-Chuan; Su, Gang

    2016-06-01

    The quantum phase transition, scaling behaviors, and thermodynamics in the spin-1/2 quantum Heisenberg model with antiferromagnetic coupling J >0 in the armchair direction and ferromagnetic interaction J'Monte Carlo method. By calculating the Binder ratio Q2 and spin stiffness ρ in two directions for various coupling ratios α =J'/J under different lattice sizes, we found that a quantum phase transition from the dimerized phase to the stripe phase occurs at the quantum critical point αc=-0.93 . Through the finite-size scaling analysis on Q2, ρx, and ρy, we determined the critical exponent related to the correlation length ν to be 0.7212(8), implying that this transition falls into a classical Heisenberg O(3) universality. A zero magnetization plateau is observed in the dimerized phase, whose width decreases with increasing α . A phase diagram in the coupling ratio α -magnetic field h plane is obtained, where four phases, including dimerized, stripe, canted stripe, and polarized, are identified. It is also unveiled that the temperature dependence of the specific heat C (T ) for different α 's intersects precisely at one point, similar to that of liquid 3He under different pressures and several magnetic compounds under various magnetic fields. The scaling behaviors of Q2, ρ , and C (T ) are carefully analyzed. The susceptibility is compared with the experimental data to give the magnetic parameters of both compounds.

  14. Correlation between exchange bias and pinned interfacial spins.

    Science.gov (United States)

    Ohldag, H; Scholl, A; Nolting, F; Arenholz, E; Maat, S; Young, A T; Carey, M; Stöhr, J

    2003-07-04

    Using x-ray magnetic circular dichroism, we have detected the very interfacial spins that are responsible for the horizontal loop shift in three different exchange bias sandwiches, chosen because of their potential for device applications. The "pinned" uncompensated interfacial spins constitute only a fraction of a monolayer and do not rotate in an external magnetic field since they are tightly locked to the antiferromagnetic lattice. A simple extension of the Meiklejohn and Bean model is proposed to account quantitatively for the exchange bias fields in the three studied systems from the experimentally determined number of pinned moments and their sizes.

  15. Nonlinear magnetization dynamics of antiferromagnetic spin resonance induced by intense terahertz magnetic field

    CERN Document Server

    Mukai, Y; Yamamoto, T; Kageyama, H; Tanaka, K

    2016-01-01

    We report on the nonlinear magnetization dynamics of a HoFeO3 crystal induced by a strong terahertz magnetic field resonantly enhanced with a split ring resonator and measured with magneto-optical Kerr effect microscopy. The terahertz magnetic field induces a large change (~40%) in the spontaneous magnetization. The frequency of the antiferromagnetic resonance decreases in proportion to the square of the magnetization change. A modified Landau-Lifshitz-Gilbert equation with a phenomenological nonlinear damping term quantitatively reproduced the nonlinear dynamics.

  16. Phase diagram and spin correlations of the Kitaev-Heisenberg model: Importance of quantum effects

    Science.gov (United States)

    Gotfryd, Dorota; Rusnačko, Juraj; Wohlfeld, Krzysztof; Jackeli, George; Chaloupka, Jiří; Oleś, Andrzej M.

    2017-01-01

    We explore the phase diagram of the Kitaev-Heisenberg model with nearest neighbor interactions on the honeycomb lattice using the exact diagonalization of finite systems combined with the cluster mean field approximation, and supplemented by the insights from analytic approaches: the linear spin-wave and second-order perturbation theories. This study confirms that by varying the balance between the Heisenberg and Kitaev term, frustrated exchange interactions stabilize in this model either one of four phases with magnetic long range order: Néel phase, ferromagnetic phase, and two other phases with coexisting antiferromagnetic and ferromagnetic bonds, zigzag and stripy phase, or one of two distinct spin-liquid phases. Out of these latter disordered phases, the one with ferromagnetic Kitaev interactions has a substantially broader range of stability as the neighboring competing ordered phases, ferromagnetic and stripy, have very weak quantum fluctuations. Focusing on the quantum spin-liquid phases, we study spatial spin correlations and dynamic spin structure factor of the model by the exact diagonalization technique, and discuss the evolution of gapped low-energy spin response across the quantum phase transitions between the disordered spin liquid and phases with long range magnetic order.

  17. Current correlations in quantum spin Hall insulators.

    Science.gov (United States)

    Schmidt, Thomas L

    2011-08-26

    We consider a four-terminal setup of a two-dimensional topological insulator (quantum spin Hall insulator) with local tunneling between the upper and lower edges. The edge modes are modeled as helical Luttinger liquids and the electron-electron interactions are taken into account exactly. Using perturbation theory in the tunneling, we derive the cumulant generating function for the interedge current. We show that different possible transport channels give rise to different signatures in the current noise and current cross correlations, which could be exploited in experiments to elucidate the interplay between electron-electron interactions and the helical nature of the edge states.

  18. Pair correlation function for spin glasses

    Science.gov (United States)

    Fernández, Julio F.; Alonso, Juan J.

    2012-10-01

    We extract a pair correlation function (PCF) from probability distributions of the spin-overlap parameter q. The distributions come from Monte Carlo simulations. A measure, w, of the thermal fluctuations of magnetic patterns follows from the PCFs. We also obtain rms deviations (over different system samples) δp away from average probabilities for q. For the linear system sizes L that we have studied, w and δp are independent of L in the Edwards-Anderson model but scale as 1/L and L, respectively, in the Sherrington-Kirkpatrick model.

  19. Spin waves and phonons in a paraelectric antiferromagnet EuTiO3

    Science.gov (United States)

    Cao, Huibo; Hong, Jiawang; Delaire, Olivier; Hahn, Steven; Ehlers, Georg; Chi, Songxue; Garlea, Vasile; Fernandez-Baca, Jaime; Chakoumakos, Bryan; Yan, Jiaqiang; Sales, Brian

    2015-03-01

    Perovskite titanates ATiO3 (A=Ba,Pb,Sr,Ca,Cd,or Eu) are widely studied for their interesting instabilities and broad applications. A ferroelectric (FE) transition occurs in Ba, Pb, and Cd titanates, but not in SrTiO3 (STO) or EuTiO3 (ETO). In the case of STO, fluctuations yield a quantum paraelectric state, but whether ETO is quantum paraelectric remains an open question. Despite a number of similarities with well-studied STO, ETO is also unique owing to the magnetic Eu ions. By applying a tuning parameter, such as bi-axial tension, ETO can be turned into a FE ferromagnet, the ideal multiferroic. [J. H. Lee, et al., Nature 466, 954 (2010)] Studies of spin-spin and spin-lattice couplings in ETO are of great interest not only from a fundamental standpoint, but also for technological applications. We successfully grew a large, high-quality isotopically-enriched ETO crystal for neutron scattering. The crystal and magnetic structures were characterized with single crystal diffraction at HB-3A at HFIR at ORNL. The spin waves and phonons were measured in the temperature range of 1.5-400 K with CNCS at SNS and HB-3 at HFIR at ORNL. In this presentation, we will discuss structural instabilities, spin-spin interactions, and spin-phonon couplings in ETO. This work was supported by Office of Basic Energy Sciences, U.S. Department of Energy.

  20. Spin-noise correlations and spin-noise exchange driven by low-field spin-exchange collisions

    Science.gov (United States)

    Dellis, A. T.; Loulakis, M.; Kominis, I. K.

    2014-09-01

    The physics of spin-exchange collisions have fueled several discoveries in fundamental physics and numerous applications in medical imaging and nuclear magnetic resonance. We report on the experimental observation and theoretical justification of spin-noise exchange, the transfer of spin noise from one atomic species to another. The signature of spin-noise exchange is an increase of the total spin-noise power at low magnetic fields, on the order of 1 mG, where the two-species spin-noise resonances overlap. The underlying physical mechanism is the two-species spin-noise correlation induced by spin-exchange collisions.

  1. Quantum Entanglement in Heisenberg Antiferromagnets

    CERN Document Server

    Subramanian, V

    2004-01-01

    Entanglement sharing among pairs of spins in Heisenberg antiferromagnets is investigated using the concurrence measure. For a nondegenerate S=0 ground state, a simple formula relates the concurrence to the diagonal correlation function. The concurrence length is seen to be extremely short. A few finite clusters are studied numerically, to see the trend in higher dimensions. It is argued that nearest-neighbour concurrence is zero for triangular and Kagome lattices. The concurrences in the maximal-spin states are explicitly calculated, where the concurrence averaged over all pairs is larger than the S=0 states.

  2. Ferrimagnetic and Long Period Antiferromagnetic Phases in High Spin Heisenberg Chains with D-Modulation

    Science.gov (United States)

    Hida, Kazuo

    2007-02-01

    The ground state properties of the high spin Heisenberg chains with alternating single site anisotropy are investigated by means of the numerical exact daigonaization and DMRG method. It is found that the ferrimagnetic state appears between the Haldane phase and period doubled Néel phase for the integer spin chains. On the other hand, the transition from the Tomonaga-Luttinger liquid state into the ferrimagnetic state takes place for the half-odd-integer spin chains. In the ferrimagnetic phase, the spontaneous magnetization varies continuously with the modulation amplitude of the single site anisotropy. Eventually, the magnetization is locked to fractional values of the saturated magnetization. These fractional values satisfy the Oshikawa-Yamanaka-Affleck condition. The local spin profile is calculated to reveal the physical nature of each state. In contrast to the case of frustration induced ferrimagnetism, no incommensurate magnetic superstructure is found.

  3. Single-pulse terahertz coherent control of spin resonance in the canted antiferromagnet YFeO3, mediated by dielectric anisotropy

    DEFF Research Database (Denmark)

    Jin, Zuanming; Mics, Zoltán; Ma, Guohong;

    2013-01-01

    We report on the coherent control of terahertz (THz) spin waves in a canted antiferromagnet yttrium orthoferrite, YFeO3, associated with a quasiferromagnetic (quasi-FM) spin resonance at a frequency of 0.3 THz, using a single-incident THz pulse. The spin resonance is excited impulsively...... by the magnetic field component of the THz pulse. The intrinsic dielectric anisotropy of YFeO3 in the THz range allows for coherent control of both the amplitude and the phase of the excited spin wave. The coherent control is based on simultaneous generation of two interfering phase-shifted spin waves whose...... amplitudes and relative phase, dictated by the dielectric anisotropy of the YFeO3 crystal, can be controlled by varying the polarization of the incident THz pulse with respect to the crystal axes. The spatially anisotropic decay of the THz-excited FM spin resonance in YFeO3, leading to an increasingly linear...

  4. Thermal form factor approach to the ground-state correlation functions of the XXZ chain in the antiferromagnetic massive regime

    CERN Document Server

    Dugave, Maxime; Kozlowski, Karol K; Suzuki, Junji

    2016-01-01

    We use the form factors of the quantum transfer matrix in the zero-temperature limit in order to study the two-point ground-state correlation functions of the XXZ chain in the antiferromagnetic massive regime. We obtain novel form factor series representations of the correlation functions which differ from those derived either from the q-vertex-operator approach or from the algebraic Bethe Ansatz approach to the usual transfer matrix. We advocate that our novel representations are numerically more efficient and allow for a straightforward calculation of the large-distance asymptotic behaviour of the two-point functions. Keeping control over the temperature corrections to the two-point functions we see that these are of order $T^\\infty$ in the whole antiferromagnetic massive regime. The isotropic limit of our result yields a novel form factor series representation for the two-point correlation functions of the XXX chain at zero magnetic field.

  5. Spin freezing in the pyrochlore antiferromagnet Pr{sub 2}Zr{sub 2}O{sub 7}

    Energy Technology Data Exchange (ETDEWEB)

    Matsuhira, K; Takagi, S [Department of Electronics, Faculty of Engineering, Kyushu Institute of Technology, Kitakyushu 804-8550 (Japan); Sekine, C [Muroran Institute of Technology, Muroran 050-8585 (Japan); Paulsen, C [Institute Neel C.N.R.S - Universite Joseph Fourier, BP 166, 38042, Grenoble (France); Wakeshima, M; Hinatsu, Y [Graduate School of Science, Hokkaido University, Sapporo 060-0810 (Japan); Kitazawa, T; Kiuchi, Y; Hiroi, Z, E-mail: matuhira@elcs.kyutech.ac.j [Institute for Solid State Physics, University of Tokyo, Kashiwa 277-8581 (Japan)

    2009-01-01

    We report on the low temperature magnetism of pyrochlore oxide Pr{sub 2}Zr{sub 2}O{sub 7}. The crystal electric field ground state in Pr{sup 3+} (4f{sup 2}, J = 4) ions has non-Kramers doublet with local <111> Ising magnetic anisotropy. The negative Curie-Weiss temperature below 10 K (-0.55 K) indicates an antiferromagnetic coupling between the spins. The AC magnetic susceptibility does not exhibit any long range ordering at least down to 76 mK. Instead, a frequency dependence of AC magnetic susceptibility is observed below 0.3 K, indicating a spin freezing behavior. Furthermore, recently we have succeeded for the first time in growing a single crystal of Pr{sub 2}Zr{sub 2}O{sub 7} by the floating-zone method using an infrared furnace equipped with four Xe lamps. We will also comment on the crystal growth of Pr{sub 2}Zr{sub 2}O{sub 7}.

  6. Ground States of Spin-1/2 Heisenberg Antiferromagnets with Frustration on a Diamond-Like-Decorated Square Lattice

    Science.gov (United States)

    Hirose, Yuhei; Oguchi, Akihide; Fukumoto, Yoshiyuki

    2017-01-01

    We study the ground-state phase diagram of a Heisenberg model with spin S = 1/2 on a diamond-like-decorated square lattice. A diamond unit has two types of antiferromagnetic exchange interactions, and the ratio λ of the length of the diagonal bond to that of the other four edges determines the strength of frustration. It has been pointed out [https://doi.org/10.7566/JPSJ.85.033705" xlink:type="simple">J. Phys. Soc. Jpn 85, 033705 (2016)] that the so-called tetramer-dimer states, which are expected to be stabilized in an intermediate region of λc < λ < 2, are identical to the square-lattice dimer-covering states, which ignited renewed interest in high-dimensional diamond-like-decorated lattices. In order to determine the phase boundary λc, we employ the modified spin wave method to estimate the energy of the ferrimagnetic state and obtain λc = 0.974. Furthermore, our numerical diagonalization study suggests that other cluster states do not appear in the ground-state phase diagram.

  7. Fermi surface evolution and checker-board block-spin antiferromagnetism in AxFe2-ySe2

    Science.gov (United States)

    Tai, Yuan-Yen; Zhu, Jian-Xin; Graf, Matthias J.; Ting, C. S.

    2012-10-01

    We develop an effective multiorbital mean-field t-J Hamiltonian with realistic tight-binding and exchange parameters to describe the electronic and magnetic structures of iron-selenide based superconductors AxFe2-ySe2 for iron vacancy doping in the range 0≤y≤0.4. The Fermi surface topology extracted from the spectral function of angle-resolved photoemission spectroscopy (ARPES) experiments is adequately accounted for by a tight-binding lattice model with random vacancy disorder. Since introducing iron vacancies breaks the lattice periodicity of the stochiometric compound, it greatly affects the electronic band structure. With changing vacancy concentration, the electronic band structure evolves, leading to a reconstruction of the Fermi surface topology. For intermediate doping levels, the realized stable electronic structure is a compromise between the solutions for the perfect lattice with y=0 and the vacancy stripe-ordered lattice with y=0.4, which results in a competition between vacancy random disorder and vacancy stripe order. A multiorbital hopping model is parameterized by comparing Fermi surface topologies to ARPES experiments, from which we construct a mean-field t-J lattice model to study the paramagnetic and antiferromagnetic (AFM) phases of K0.8Fe1.6Se2. In the AFM phase the calculated spin magnetization of the t-J model leads to a checker-board block-spin structure in good agreement with neutron scattering experiments and abinitio calculations.

  8. Anomalous curie response of impurities in quantum-critical spin-1/2 Heisenberg antiferromagnets.

    Science.gov (United States)

    Höglund, Kaj H; Sandvik, Anders W

    2007-07-13

    We consider a magnetic impurity in two different S=1/2 Heisenberg bilayer antiferromagnets at their respective critical interlayer couplings separating Néel and disordered ground states. We calculate the impurity susceptibility using a quantum Monte Carlo method. With intralayer couplings in only one of the layers (Kondo lattice), we observe an anomalous Curie constant C*, as predicted on the basis of field-theoretical work [S. Sachdev, Science 286, 2479 (1999)10.1126/science.286.5449.2479]. The value C* = 0.262 +/- 0.002 is larger than the normal Curie constant C=S(S+1)/3. Our low-temperature results for a symmetric bilayer are consistent with a universal C*.

  9. Variational Monte Carlo study of chiral spin liquid in quantum antiferromagnet on the triangular lattice

    Science.gov (United States)

    Hu, Wen-Jun; Gong, Shou-Shu; Sheng, D. N.

    2016-08-01

    By using Gutzwiller projected fermionic wave functions and variational Monte Carlo technique, we study the spin-1 /2 Heisenberg model with the first-neighbor (J1), second-neighbor (J2), and additional scalar chiral interaction JχSi.(Sj×Sk) on the triangular lattice. In the nonmagnetic phase of the J1-J2 triangular model with 0.08 ≲J2/J1≲0.16 , recent density-matrix renormalization group (DMRG) studies [Zhu and White, Phys. Rev. B 92, 041105(R) (2015), 10.1103/PhysRevB.92.041105 and Hu, Gong, Zhu, and Sheng, Phys. Rev. B 92, 140403(R) (2015), 10.1103/PhysRevB.92.140403] find a possible gapped spin liquid with the signal of a competition between a chiral and a Z2 spin liquid. Motivated by the DMRG results, we consider the chiral interaction JχSi.(Sj×Sk) as a perturbation for this nonmagnetic phase. We find that with growing Jχ, the gapless U(1) Dirac spin liquid, which has the best variational energy for Jχ=0 , exhibits the energy instability towards a gapped spin liquid with nontrivial magnetic fluxes and nonzero chiral order. We calculate topological Chern number and ground-state degeneracy, both of which identify this flux state as the chiral spin liquid with fractionalized Chern number C =1 /2 and twofold topological degeneracy. Our results indicate a positive direction to stabilize a chiral spin liquid near the nonmagnetic phase of the J1-J2 triangular model.

  10. Strong anisotropic anomalous Hall effect and spin Hall effect in the chiral antiferromagnetic compounds Mn3X (X =Ge , Sn, Ga, Ir, Rh, and Pt)

    Science.gov (United States)

    Zhang, Yang; Sun, Yan; Yang, Hao; Železný, Jakub; Parkin, Stuart P. P.; Felser, Claudia; Yan, Binghai

    2017-02-01

    We have carried out a comprehensive study of the intrinsic anomalous Hall effect and spin Hall effect of several chiral antiferromagnetic compounds Mn3X (X = Ge, Sn, Ga, Ir, Rh and Pt) by ab initio band structure and Berry phase calculations. These studies reveal large and anisotropic values of both the intrinsic anomalous Hall effect and spin Hall effect. The Mn3X materials exhibit a noncollinear antiferromagnetic order which, to avoid geometrical frustration, forms planes of Mn moments that are arranged in a Kagome-type lattice. With respect to these Kagome planes, we find that both the anomalous Hall conductivity (AHC) and the spin Hall conductivity (SHC) are quite anisotropic for any of these materials. Based on our calculations, we propose how to maximize AHC and SHC for different materials. The band structures and corresponding electron filling, that we show are essential to determine the AHC and SHC, are compared for these different compounds. We point out that Mn3Ga shows a large SHC of about 600 (ℏ /e ) (Ωcm) -1 . Our work provides insights into the realization of strong anomalous Hall effects and spin Hall effects in chiral antiferromagnetic materials.

  11. Magnetic dichroism and spin structure of antiferromagnetic NiO(001) films

    NARCIS (Netherlands)

    Altieri, S; Finazzi, M; Hsieh, HH; Lin, HJ; Chen, CT; Hibma, T; Valeri, S; Sawatzky, GA

    2003-01-01

    We find that Ni L-2 edge x-ray magnetic linear dichroism is fully reversed for NiO(001) films on materials with reversed lattice mismatch. We relate this phenomenon to a preferential stabilization of magnetic S domains with main spin component either in or out of the plane, via dipolar interactions.

  12. Negative Correlations and Entanglement in Higher-Spin Dicke States

    Science.gov (United States)

    Wang, Xiaoqian; Zhong, Wei; Wang, Xiaoguang

    2016-10-01

    We consider entanglement criteria based on the spin squeezing inequalities for arbitrary spin systems. Here we use the negative correlations to detect the entanglement in the system with exchange symmetry. For arbitrary spin systems, we can find that the state is entangled, when the minimal pairwise correlation is negative. Then we give a parameter which is defined by the collective angular momentum operator, to detect the entanglement for the Dicke state with N spin -1 particles, and the results are as the same as negative correlation. We also consider the directions of negative correlation, the state is entangled in two orthogonal directions for the superposition of Dicke state without parity.

  13. Direct observation of impurity-induced magnetism in a spin-(1/2) antiferromagnetic Heisenberg two-leg spin ladder.

    Science.gov (United States)

    Casola, F; Shiroka, T; Wang, S; Conder, K; Pomjakushina, E; Mesot, J; Ott, H-R

    2010-08-06

    Nuclear magnetic resonance and magnetization measurements were used to probe the magnetic features of single-crystalline Bi(Cu(1-x)Zn(x))(2)PO(6) with 00 and we present clear evidence for a temperature-dependent variation of the local magnetization close to the Zn sites. The generic nature of this observation is indicated by results of model calculations on appropriate spin systems of limited size employing quantum Monte Carlo methods.

  14. Critical and reentrant behavior of the spin quantum 1/2 anisotropic Heisenberg antiferromagnet model with Dzyaloshinskii–Moriya interaction in a longitudinal magnetic field

    Energy Technology Data Exchange (ETDEWEB)

    Parente, Walter E.F.; Pacobahyba, J.T.M.; Araújo, Ijanílio G. [Departamento de Física, Universidade Federal de Roraima, BR 174, Km 12. Bairro Monte Cristo. CEP: 69300-000 Boa Vista, Roraima (Brazil); Neto, Minos A., E-mail: minos@pq.cnpq.br [Universidade Federal do Amazonas, Departamento de Física, 3000, Japiim, 69077-000, Manaus-AM (Brazil); Ricardo de Sousa, J. [Universidade Federal do Amazonas, Departamento de Física, 3000, Japiim, 69077-000, Manaus-AM (Brazil); National Institute of Science and Technology for Complex Systems, 3000, Japiim, 69077-000, Manaus-AM (Brazil); Akinci, Ümit [Department of Physics, Dokuz Eylül University, Tr-35160 Izmir (Turkey)

    2014-04-15

    In this paper we study the quantum spin-1/2 anisotropic Heisenberg antiferromagnet model in the presence of a Dzyaloshinskii–Moriya interaction (D) and a uniform longitudinal (H) magnetic field. Using the effective-field theory with a finite cluster N=2 spin (EFT-2) we calculate the phase diagrams in the H−T and D−T planes on a simple cubic lattice (z=6). We have only observed second order phase transitions for values between Δ∈[0,1], where the cases were analysed: Ising (Δ=1), anisotropic Heisenberg (Δ=0.6) and isotropic Heisenberg (Δ=0). - Highlights: • Anisotropic Heisenberg antiferromagnet on a simple cubic lattice. • Effective-field theory. • Dzyaloshinskii–Moriya interaction.

  15. Density matrix renormalization group numerical study of the kagome antiferromagnet.

    Science.gov (United States)

    Jiang, H C; Weng, Z Y; Sheng, D N

    2008-09-12

    We numerically study the spin-1/2 antiferromagnetic Heisenberg model on the kagome lattice using the density-matrix renormalization group method. We find that the ground state is a magnetically disordered spin liquid, characterized by an exponential decay of spin-spin correlation function in real space and a magnetic structure factor showing system-size independent peaks at commensurate magnetic wave vectors. We obtain a spin triplet excitation gap DeltaE(S=1)=0.055+/-0.005 by extrapolation based on the large size results, and confirm the presence of gapless singlet excitations. The physical nature of such an exotic spin liquid is also discussed.

  16. Similarity between the superconductivity in the graphene with the spin transport in the two-dimensional antiferromagnet in the honeycomb lattice

    Science.gov (United States)

    Lima, L. S.

    2017-02-01

    We have used the Dirac's massless quasi-particles together with the Kubo's formula to study the spin transport by electrons in the graphene monolayer. We have calculated the electric conductivity and verified the behavior of the AC and DC currents of this system, that is a relativistic electron plasma. Our results show that the AC conductivity tends to infinity in the limit ω → 0 , similar to the behavior obtained for the spin transport in the two-dimensional frustrated antiferromagnet in the honeycomb lattice. We have made a diagrammatic expansion for the Green's function and we have not gotten significative change in the results.

  17. Spin dynamics of frustrated easy-axis triangular antiferromagnet 2H-AgNiO2 explored by inelastic neutron scattering

    OpenAIRE

    Wheeler, E M; Coldea, R.; Wawrzynska, E.; Sorgel, T.; Jansen, M; Koza, M. M.; Taylor, J; Adroguer, P.; Shannon, N.

    2009-01-01

    We report inelastic neutron scattering measurements of the spin dynamics in the layered hexagonal magnet 2H-AgNiO2 which has stacked triangular layers of antiferromagnetically-coupled Ni2+ spins (S=1) ordered in a collinear alternating stripe pattern. We observe a broad band of magnetic excitations above a small gap of 1.8 meV and extending up to 7.5 meV, indicating strongly dispersive excitations. The measured dispersions of the boundaries of the powder-averaged spectrum can be quantitativel...

  18. Effect of spatial spin modulation on relaxation and NMR frequencies of sup 5 sup 7 Fe nuclei in ferroelectric antiferromagnetic BiFeO sub 3

    CERN Document Server

    Zalessky, A V; Zvezdin, A K; Gippius, A A; Morozova, E N; Khozeev, D F; Bush, A S; Pokatilov, V S

    2002-01-01

    The NMR spectra on the iron nuclei in the BiFeO sub 3 antiferromagnetic sample enriched by the sup 5 sup 7 Fe (95.43%) with the spatially-modulated magnetic structure are studied. It is established that the cycloid-type spin modulation in the BiFeO sub 3 produces spatial modulation of the nuclear spin-spin relaxation velocity and leads to the spectral nonuniform widening of the NMR local line. It is determined also that the local magnetic moments of the iron ions on various cycloid sections differently depend on temperature which testifies to different character of the spin waves excitation. The analogy of the experimental results with the NMR regularities in the Bloch wall is discussed

  19. Unusual Charge Transport and Spin Response of Doped Bilayer Triangular Antiferromagnets

    Institute of Scientific and Technical Information of China (English)

    LIANG Ying; MA Tian-Xing; FENG Shi-Ping

    2003-01-01

    Within the t-J model, the charge transport and spin response of the doped bilayer triangular antiferromagnetare studied by considering the bilayer interaction. Although the bilayer interaction leads to the band splitting in theelectronic structure, the qualitative behaviors of the physical properties are the same as in the single layer case. Theconductivity spectrum shows the low-energy peak and unusual midinfrared band, the temperature-dependent resistivityis characterized by the nonlinearity metallic-like behavior in the higher temperature range and the deviation from themetallic-like behavior in the lower temperature range and the commensurate neutron scattering peak near the half-fillingis split into six incommensurate peaks in the underdoped regime, with the incommensurability increasing with the holeconcentration at lower dopings, and saturating at higher dopings.

  20. Spin-spin correlations of magnetic adatoms on graphene

    Science.gov (United States)

    Güçlü, A. D.; Bulut, Nejat

    2015-03-01

    We study the interaction between two magnetic adatom impurities in graphene using the Anderson model. The two-impurity Anderson Hamiltonian is solved numerically by using the quantum Monte Carlo technique. We find that the interimpurity spin susceptibility is strongly enhanced at low temperatures, significantly diverging from the well-known Ruderman-Kittel-Kasuya-Yoshida result which decays as R-3.

  1. Competition between itinerant ferromagnetism and spin-density wave antiferromagnetism in FeGa

    Science.gov (United States)

    Wu, Yan; Cao, Huibo; McCandles, Gregory; Chan, Julia; Karki, Amar; Jin, Rongying; Ditusa, John

    2015-03-01

    The metallic magnetFeGadisplays a rich magnetic behavior that includes transitions between a FM ground state to a AFM intermediate state at 68 K and back to a FM state at 360 K. The phase transition at 360 K is accompanied by a discontinuous hysteretic change in the electrical resistivity. In addition, the application of moderate magnetic fields cause a sharp transformation from the AFM to FM state with a critical Hthat grows dramatically with T.To explore the cause of this unusual competition of magnetic states, we investigated the magnetic structure of FeGavia extensive single crystal neutron diffraction measurements. These measurements revealed a FM ordering with magnetic moments lying along the crystallographic c-axis both below 68 K and above 360 K as well as incommensurate spin density wave order between these temperatures. Our refinement of the diffraction data has uncovered the existence of a small non-coplanar moment which may be the origin of our previously discovered topological Hall Effect.

  2. Spin correlations in Ho2Ti2O7: A dipolar spin ice system

    DEFF Research Database (Denmark)

    Bramwell, S.T.; Harris, M.J.; Hertog, B.C. den;

    2001-01-01

    The pyrochlore material Ho(2)Ti(2)O(7) has been suggested to show "spin ice" behavior. We present neutron scattering and specific heat results that establish unambiguously that Ho(2)Ti(2)O(7) exhibits spin ice correlations at low temperature. Diffuse magnetic neutron scattering is quite well...... described by a nearest neighbor spin ice model and very accurately described by a dipolar spin ice model. The heat capacity is well accounted for by the sum of a dipolar spin ice contribution and an expected nuclear spin contribution, known to exist in other Ho(3+) salts. These results settle the question...... of the nature of the low temperature spin correlations in Ho(2)Ti(2)O(7) for which contradictory claims have been made....

  3. Evidence for stripe correlations of spins and holes in copper oxide superconductors

    Science.gov (United States)

    Tranquada, J. M.; Sternlieb, B. J.; Axe, J. D.; Nakamura, Y.; Uchida, S.

    1995-06-01

    ONE of the long-standing mysteries associated with the high-temperature copper oxide superconductors concerns the anomalous suppression1 of superconductivity in La2-xBaxCuO4 (and certain related compounds) when the hole concentration x is near ⅛. Here we examine the possibility that this effect is related to dynamical two-dimensional spin correlations, incommensurate with the crystal lattice, that have been observed in La2-xSrxCuO4 by neutron scattering2 4. A possible explanation for the incommensurability involves a coupled, dynamical modulation of spin and charge in which antiferromagnetic 'stripes' of copper spins are separated by periodically spaced domain walls to which the holes segregate5 9. An ordered stripe phase of this type has recently been observed in hole-doped La2NiO4 (refs 10 12). We present evidence from neutron diffraction that in the copper oxide material La1.6-xNd0.4SrxCuO4, with x = 0.12, a static analogue of the dynamical stripe phase is present, and is associated with an anomalous suppression of superconductivity13,14. Our results thus provide an explanation of the '⅛' conundrum, and also support the suggestion15 that spatial modulations of spin and charge density are related to superconductivity in the copper oxides.

  4. Direct measurement of antiferromagnetic domain fluctuations.

    Energy Technology Data Exchange (ETDEWEB)

    Shpyrko, O. G.; Isaacs, E. D.; Logan, J. M.; Feng, Y.; Aeppli, G.; Jaramillo, R.; Kim, H. C.; Rosenbaum, T. F.; Zschack, P.; Sprung, M.; Narayanan, S.; Sandy, A.; Univ. of Chicago; Univ. College London

    2007-05-03

    Measurements of magnetic noise emanating from ferromagnets owing to domain motion were first carried out nearly 100 years ago1, and have underpinned much science and technology2, 3. Antiferromagnets, which carry no net external magnetic dipole moment, yet have a periodic arrangement of the electron spins extending over macroscopic distances, should also display magnetic noise. However, this must be sampled at spatial wavelengths of the order of several interatomic spacings, rather than the macroscopic scales characteristic of ferromagnets. Here we present a direct measurement of the fluctuations in the nanometer-scale superstructure of spin- and charge-density waves associated with antiferromagnetism in elemental chromium. The technique used is X-ray photon correlation spectroscopy, where coherent X-ray diffraction produces a speckle pattern that serves as a 'fingerprint' of a particular magnetic domain configuration. The temporal evolution of the patterns corresponds to domain walls advancing and retreating over micrometer distances. This work demonstrates a useful measurement tool for antiferromagnetic domain wall engineering, but also reveals a fundamental finding about spin dynamics in the simplest antiferromagnet: although the domain wall motion is thermally activated at temperatures above 100 K, it is not so at lower temperatures, and indeed has a rate that saturates at a finite value--consistent with quantum fluctuations--on cooling below 40 K.

  5. Thermal form factor approach to the ground-state correlation functions of the XXZ chain in the antiferromagnetic massive regime

    Science.gov (United States)

    Dugave, Maxime; Göhmann, Frank; Kozlowski, Karol K.; Suzuki, Junji

    2016-09-01

    We use the form factors of the quantum transfer matrix in the zero-temperature limit in order to study the two-point ground-state correlation functions of the XXZ chain in the antiferromagnetic massive regime. We obtain novel form factor series representations of the correlation functions which differ from those derived either from the q-vertex-operator approach or from the algebraic Bethe Ansatz approach to the usual transfer matrix. We advocate that our novel representations are numerically more efficient and allow for a straightforward calculation of the large-distance asymptotic behaviour of the two-point functions. Keeping control over the temperature corrections to the two-point functions we see that these are of order {T}∞ in the whole antiferromagnetic massive regime. The isotropic limit of our result yields a novel form factor series representation for the two-point correlation functions of the XXX chain at zero magnetic field. Dedicated to the memory of Petr Petrovich Kulish.

  6. Non-linear spin wave theory results for the frustrated [Formula: see text] Heisenberg antiferromagnet on a body-centered cubic lattice.

    Science.gov (United States)

    Majumdar, Kingshuk; Datta, Trinanjan

    2009-10-07

    At zero temperature the sublattice magnetization of the quantum spin- 1/2 Heisenberg antiferromagnet on a body-centered cubic lattice with competing first and second neighbor exchange (J(1) and J(2)) is investigated using the non-linear spin wave theory. The zero temperature phases of the model consist of a two sublattice Néel phase for small J(2) (AF(1)) and a collinear phase at large J(2) (AF(2)). We show that quartic corrections due to spin wave interactions enhance the sublattice magnetization in both the AF(1) and the AF(2) phase. The magnetization corrections are prominent near the classical transition point of the model and in the J(2)>J(1) regime. The ground state energy with quartic interactions is also calculated. It is found that up to quartic corrections the first order phase transition (previously observed in this model) between the AF(1) and the AF(2) phase survives.

  7. 0- and 2/3-magnetization plateaus in three-leg antiferromagnetic Heisenberg spin-1/2 ladders with leg-dimerization

    Energy Technology Data Exchange (ETDEWEB)

    Li, Rui-Xue; Wang, Shu-Ling; Ni, Yun [School of Physics and Wuhan National High Magnetic Field Center, Huazhong University of Science and Technology, Wuhan 430074 (China); Yao, Kai-Lun, E-mail: klyao@mail.hust.edu.cn [School of Physics and Wuhan National High Magnetic Field Center, Huazhong University of Science and Technology, Wuhan 430074 (China); International Center of Materials Physics, Chinese Academy of Sciences, Shenyang 110015 (China); Fu, Hua-Hua [School of Physics and Wuhan National High Magnetic Field Center, Huazhong University of Science and Technology, Wuhan 430074 (China)

    2014-02-01

    Magnetic properties of three-leg antiferromagnetic Heisenberg spin-1/2 ladders with different dimerization patterns have been studied using the bond mean-field theory. Our results show that rung-columnar ladders are thermodynamically stable states for large rung-to-leg coupling ratios. Magnetization curves of leg-columnar and leg-staggered ladders always exhibit 0- and 2/3-magnetization plateaus, which do not appear in rung-columnar and rung-staggered ladders. In leg-dimerized ladders, the formation of spin dimers in the three legs results in the appearance of the 0- and 2/3-magnetization plateaus. Spin configuration in the 2/3-magnetization plateau can be understood from the mean-field bond parameters.

  8. The NQR observation of spin-Peierls transition in an antiferromagnetic MX-chain complex [NiBr(chxn)2]Br2.

    Science.gov (United States)

    Takaishi, Shinya; Tobu, Yasuhiro; Kitagawa, Hiroshi; Goto, Atsushi; Shimizu, Tadashi; Okubo, Takashi; Mitani, Tadaoki; Ikeda, Ryuichi

    2004-02-18

    81Br Nuclear quadrupole resonance (NQR) measurement was performed in an S = 1/2 one-dimensional Heisenberg antiferromagnetic metal complex [NiBr(chxn)2]Br2 (chxn: 1R,2R-diaminocyclohexane), having a halogen-bridged MX chain structure -Br-Ni3+-Br-Ni3+-Br-. Two 81Br NQR signals were observed below 40 K, while a single signal was observed above 130 K, showing the presence of two nonequivalent bridging Br sites below 40 K. This NQR result together with previously reported magnetic susceptibility and X-ray results indicate the occurrence of a transition into a spin-Peierls state between 40 and 130 K. This communication reports the first spin-Peierls transition in metal complexes in which pure d electrons contribute to the magnetism. In addition, we demonstrated a new experimental method for studying a spin-Peierls system.

  9. Quantification of quantum discord in a antiferromagnetic Heisenberg compound

    Energy Technology Data Exchange (ETDEWEB)

    Singh, H., E-mail: chiranjib@iiserkol.ac.in; Chakraborty, T., E-mail: chiranjib@iiserkol.ac.in; Mitra, C., E-mail: chiranjib@iiserkol.ac.in [Indian Institute of Science Education and Research (IISER) Kolkata, Mohanpur Campus, Mohanpur -741252, Nadia, West Bengal (India)

    2014-04-24

    An experimental quantification of concurrence and quantum discord from heat capacity (C{sub p}) measurement performed over a solid state system has been reported. In this work, thermodynamic measurements were performed on copper nitrate (CN, Cu(NO{sub 3}){sub 2}⋅2.5H{sub 2}O) single crystals which is an alternating antiferromagnet Heisenberg spin 1/2 system. CN being a weak dimerized antiferromagnet is an ideal system to investigate correlations between spins. The theoretical expressions were used to obtain concurrence and quantum discord curves as a function of temperature from heat capacity data of a real macroscopic system, CN.

  10. Correlation Theory of the Heisenberg Antiferromagnet and Ferromagnet: Dependence on Dimension, Field, and Temperature

    DEFF Research Database (Denmark)

    Lindgård, Per-Anker

    1984-01-01

    -phase approximation and is applicable to the quantum spin case for any dimension and temperature. The static susceptibilities and the excitation spectrum are calculated. Besides the spin-wave excitations a central peak is found which can be understood as coming from local longitudinal fluctuations. The results...

  11. Effect of grain size on charge and spin correlations in Bi0.5Ca0.5MnO3 manganite nanoparticles

    Science.gov (United States)

    Ade, Ramesh; Singh, Rajender

    2016-11-01

    In this work we report the electron spin resonance (ESR) and magnetization (M) studies to understand the effect of grain size (GS) on the charge ordering and spin correlations in Bi0.5Ca0.5MnO3 manganite synthesized by sol-gel method. The suppression of charge ordering (CO), long-range antiferromagnetic (AFM) state, shifting of ferromagnetic (FM)-cluster glass (CG) transition towards higher temperatures and evolution of different magnetic correlations with decrease in GS are discussed in view of the changes in surface to volume ratio of nano-grains.

  12. Quantum-spin-liquid states in the two-dimensional kagome antiferromagnets ZnxCu4-x(OD)6Cl2.

    Science.gov (United States)

    Lee, S-H; Kikuchi, H; Qiu, Y; Lake, B; Huang, Q; Habicht, K; Kiefer, K

    2007-11-01

    A three-dimensional system of interacting spins typically develops static long-range order when it is cooled. If the spins are quantum (S=1/2), however, novel quantum paramagnetic states may appear. The most highly sought state among them is the resonating-valence-bond state, in which every pair of neighbouring quantum spins forms an entangled spin singlet (valence bonds) and these singlets are quantum mechanically resonating among themselves. Here we provide an experimental indication for such quantum paramagnetic states existing in frustrated antiferromagnets, Zn(x)Cu(4-x)(OD)(6)Cl(2), where the S=1/2 magnetic Cu2+ moments form layers of a two-dimensional kagome lattice. We find that in Cu(4)(OD)(6)Cl(2), where distorted kagome planes are weakly coupled, a dispersionless excitation mode appears in the magnetic excitation spectrum below approximately 20 K, whose characteristics resemble those of quantum spin singlets in a solid state, known as a valence-bond solid, that breaks translational symmetry. Doping with non-magnetic Zn2+ ions reduces the distortion of the kagome lattice, and weakens the interplane coupling but also dilutes the magnetic occupancy of the kagome lattice. The valence-bond-solid state is suppressed, and for ZnCu(3)(OD)(6)Cl(2), where the kagome planes are undistorted and 90% occupied by the Cu2+ ions, the low-energy spin fluctuations become featureless.

  13. Reentrant phenomenon and inverse magnetocaloric effect in a generalized spin-(1/2,  s) Fisher’s super-exchange antiferromagnet

    Science.gov (United States)

    Gálisová, Lucia

    2016-11-01

    The thermodynamic and magnetocaloric properties of a generalized spin-(1/2,  s) Fisher’s super-exchange antiferromagnet are investigated precisely by using the decoration-iteration mapping transformation. Besides the critical temperature, sublattice magnetization, total magnetization, entropy and specific heat, the isothermal entropy change and adiabatic temperature change are also rigorously calculated in order to examine the cooling efficiency of the model in the vicinity of the first- and second-order phase transitions. It is shown that an enhanced inverse magnetocaloric effect occurs around the temperature interval {{T}\\text{c}}(B\

  14. Spin-polarized calculations of electronic structures in ferromagnetic and antiferromagnetic Zn{sub 0.75}TM{sub 0.25}Se (TM=Cr, Fe, Co and Ni)

    Energy Technology Data Exchange (ETDEWEB)

    Amari, S., E-mail: siham_amari@yahoo.fr [Laboratoire de Modelisation et de Simulation en Sciences des Materiaux, Departement de Physique Universite Djillali Liabes, Sidi Bel-Abbes (Algeria); Mecabih, S.; Abbar, B.; Bouhafs, B. [Laboratoire de Modelisation et de Simulation en Sciences des Materiaux, Departement de Physique Universite Djillali Liabes, Sidi Bel-Abbes (Algeria)

    2012-09-15

    In this work, we aim to examine the spin-polarized electronic band structures, the local densities of states as well as the magnetism of Zn{sub 1-x}TM{sub x}Se (TM=Cr, Fe, Co and Ni) diluted magnetic semiconductors in the ferromagnetic (FM) and antiferromagnetic (AFM) phases, and with 25% of TM. The calculations are performed by the developed full-potential augmented plane wave plus local orbitals method within the spin density functional theory. As exchange-correlation potential we used the generalized gradient approximation (GGA) form. We treated the ferromagnetic and antiferromagnetic phases and we found that all compounds are stable in the ferromagnetic structure. Structural properties are computed after total energy minimization. Our results show that the cohesive energies of Zn{sub 0.75}TM{sub 0.25}Se are greater than that of zinc blende ZnSe. We discuss the electronic structures, total and partial densities of states, local moments and the p-d exchange splitting. Furthermore, we found that p-d hybridization reduces the local magnetic moment of TM and produces small local magnetic moments on the nonmagnetic Zn and Se sites. We found also that in the AFM phase the TM local magnetic moments are smaller than in the FM phase; this is due to the greater interaction of the TM d-up and d-down orbitals. - Highlights: Black-Right-Pointing-Pointer The calculation of the exchange constants of ZnTMSe (TM=Cr, Fe, Co and Ni). Black-Right-Pointing-Pointer Prediction of the spin-exchange splitting of ZnTMSe (TM=Cr, Fe, Co and Ni). Black-Right-Pointing-Pointer The study of ZnTMSe diluted magnetic semiconductors in the FM and AFM phases.

  15. CP-sensitive spin-spin correlations in neutralino production at the ILC

    Science.gov (United States)

    Bartl, A.; Hohenwarter-Sodek, K.; Kernreiter, T.; Kittel, O.; Terwort, M.

    2009-07-01

    We study the CP-violating terms of the spin-spin correlations in neutralino production and their subsequent two-body decays into sleptons plus leptons at the ILC. We analyze CP-sensitive observables with the help of T-odd products of the spin-spin terms. These terms depend on the polarizations of both neutralinos, with one polarization perpendicular to the production plane. We present a detailed numerical study of the CP-sensitive observables, cross sections, and neutralino branching ratios in the Minimal Supersymmetric Standard Model with complex parameters.

  16. CP-sensitive spin-spin correlations in neutralino production at the ILC

    CERN Document Server

    Bartl, A; Kernreiter, T; Kittel, O; Terwort, M

    2009-01-01

    We study the CP-violating terms of the spin-spin correlations in neutralino production and their subsequent two-body decays into sleptons plus leptons at the ILC. We analyze CP-sensitive observables with the help of T-odd products of the spin-spin terms. These terms depend on the polarizations of both neutralinos, with one polarization perpendicular to the production plane. We present a detailed numerical study of the CP-sensitive observables, cross sections, and neutralino branching ratios in the Minimal Supersymmetric Standard Model with complex parameters.

  17. Spin-liquid polymorphism in a correlated electron system on the threshold of superconductivity.

    Science.gov (United States)

    Zaliznyak, Igor; Savici, Andrei T; Lumsden, Mark; Tsvelik, Alexei; Hu, Rongwei; Petrovic, Cedomir

    2015-08-18

    We report neutron scattering measurements which reveal spin-liquid polymorphism in an "11" iron chalcogenide superconductor. It occurs when a poorly metallic magnetic state of FeTe is tuned toward superconductivity by substitution of a small amount of tellurium with isoelectronic sulfur. We observe a liquid-like magnetic response, which is described by the coexistence of two disordered magnetic phases with different local structures whose relative abundance depends on temperature. One is the ferromagnetic (FM) plaquette phase observed in undoped, nonsuperconducting FeTe, which preserves the C4 symmetry of the underlying square lattice and is favored at high temperatures, whereas the other is the antiferromagnetic plaquette phase with broken C4 symmetry, which emerges with doping and is predominant at low temperatures. These findings suggest the coexistence of and competition between two distinct liquid states, and a liquid-liquid phase transformation between these states, in the electronic spin system of FeTe(1-x)(S,Se)(x). We have thus discovered the remarkable physics of competing spin-liquid polymorphs in a correlated electron system approaching superconductivity. Our results facilitate an understanding of large swaths of recent experimental data in unconventional superconductors. In particular, the phase with lower C2 local symmetry, whose emergence precedes superconductivity, naturally accounts for a propensity for forming electronic nematic states which have been observed experimentally, in cuprate and iron-based superconductors alike.

  18. NMR studies of spin dynamics in the quasi-2D square-lattice heisenberg antiferromagnet Sr sub 2 CuO sub 2 Cl sub 2

    CERN Document Server

    Suh, B J

    2000-01-01

    A comprehensive analysis of the sup 3 sup 5 Cl nuclear magnetic resonance (NMR) relaxation data in Sr sub 2 CuO sub 2 Cl sub 2 single crystals is presented. Both the spin-lattice relaxation rate, T sub 1 sup - sup 1 (=2W), and the spin-spin relaxation rate, T sub 2 sup - sup 1 , show a crossover of the spin dimensionality well above the Neel temperature T sub N. The crossover is due to easy-plane anisotropy and is apparently signaled by the partial suppression of the Cu sup 2 sup + spin fluctuations along the tetragonal c-axis. By analyzing 2W for H ll c in terms of the critical behavior of the spin correlation length, we estimate the temperature for the crossover of the Cu sup 2 sup + spin correlations from Heisenberg to XY-like behavior to be T approx =290 K.

  19. Quantum Monte Carlo Study of Random Antiferromagnetic Heisenberg Chain

    OpenAIRE

    Todo, Synge; Kato, Kiyoshi; Takayama, Hajime

    1998-01-01

    Effects of randomness on the spin-1/2 and 1 antiferromagnetic Heisenberg chains are studied using the quantum Monte Carlo method with the continuous-time loop algorithm. We precisely calculated the uniform susceptibility, string order parameter, spatial and temporal correlation length, and the dynamical exponent, and obtained a phase diagram. The generalization of the continuous-time loop algorithm for the systems with higher-S spins is also presented.

  20. Neutron scattering studies of three one-dimensional antiferromagnets

    CERN Document Server

    Kenzelmann, M

    2001-01-01

    observed in the disordered phase of spin-1/2 chains. The magnetic order of the one-dimensional spin-1/2 XY antiferromagnet Cs sub 2 CoCl sub 4 was investigated using neutron diffraction. The magnetic structure has an ordering wave-vector (0, 0.5, 0.5) for T < 217 mK and the magnetic structure is a non-linear structure with the magnetic moments at a small angle to the b axis. Above a field of H = 2.1 T the magnetic order collapses in an apparent first order phase transition, suggesting a transition to a spin-liquid phase. Low-dimensional magnets with low-spin quantum numbers are ideal model systems for investigating strongly interacting macroscopic quantum ground states and their non-linear spin excitations. This thesis describes neutron scattering experiments of three one-dimensional low-spin antiferromagnets where strong quantum fluctuations lead to highly-correlated ground states and unconventional cooperative spin excitations. The excitation spectrum of the antiferromagnetic spin-1 Heisenberg chain CsNi...

  1. The quantum spin-1/2 J1-J2 antiferromagnet on a stacked square lattice: a study of effective-field theory in a finite cluster.

    Science.gov (United States)

    Nunes, Wagner A; de Sousa, J Ricardo; Viana, J Roberto; Richter, J

    2010-04-14

    The ground state phase diagram of the quantum spin-1/2 Heisenberg antiferromagnet in the presence of nearest-neighbor (J(1)) and next-nearest-neighbor (J(2)) interactions (J(1)-J(2) model) on a stacked square lattice, where we introduce an interlayer coupling through nearest-neighbor bonds of strength J(), is studied within the framework of the differential operator technique. The Hamiltonian is solved by effective-field theory in a cluster with N=4 spins (EFT-4). We obtain the sublattice magnetization m(A) for the ordered phases: antiferromagnetic (AF) and collinear (CAF-collinear antiferromagnetic). We propose a functional for the free energy Ψ(μ)(m(μ)) (μ=A, B) to obtain the phase diagram in the λ-α plane, where λ=J()/J(1) and α=J(2)/J(1). Depending on the values of λ and α, we found different ordered states (AF and CAF) and a disordered state (quantum paramagnetic (QP)). For an intermediate region α(1c)(λ) α(2c)(λ), and below λ(1), we have the AF and CAF semi-classically ordered states, respectively. At α=α(1c)(λ) a second-order transition between the AF and QP states occurs and at α=α(2c)(λ) a first-order transition between the AF and CAF phases takes place. The boundaries between these ordered phases merge at the critical end point CEP≡(λ(1), α(c)), where α(c)≈0.56. Above this CEP there is again a direct first-order transition between the AF and CAF phases, with a behavior described by the point α(c) independent of λ ≥ λ(1).

  2. Spin-disordered superfluid state for spin-1 bosons with fractional spin and statistics

    OpenAIRE

    2002-01-01

    We study a strongly correlated spin-1 Bose gas in 2D space by using the projective construction. A spin-disordered superfluid state is constructed and proposed as a candidate competing with the conventional polar condensate when interaction is antiferromagnetic. This novel state has a non-trivial topological order whose low energy excitations carry fractional spin, charge, and statistics. The spin excitations become gapless only at the edge and are described by level-1 SU(2) Kac-Moody algebra...

  3. Mobility of the Doped Holes and the Antiferromagnetic Correlations in Underdoped High-T{sub c} Cuprates

    Energy Technology Data Exchange (ETDEWEB)

    Ando, Yoichi; Lavrov, A. N.; Komiya, Seiki; Segawa, Kouji; Sun, X. F.

    2001-07-02

    The emergence and the evolution of the metallic charge transport in the La{sub 2{minus}x}Sr {sub x}CuO{sub 4} system from lightly to optimally doped samples (x=0.01{endash}0.17 ) are studied. We demonstrate that in high-quality single crystals the in-plane resistivity shows a metallic behavior for all values of x at moderate temperatures and that the hole mobility at 300K changes only by a factor of 3 from x=0.01 to 0.17, where its x dependence is found to be intriguingly similar to that of the inverse antiferromagnetic correlation length. We discuss an incoherent-metal picture and a charged-stripe scenario as candidates to account for these peculiar features.

  4. Galaxy Zoo: Chiral correlation function of galaxy spins

    CERN Document Server

    Slosar, Anze; Bamford, Steven; Lintott, Chris; Andreescu, Dan; Murray, Phil; Nichol, Robert; Raddick, M Jordan; Schawinski, Kevin; Szalay, Alex; Thomas, Daniel; Vandenberg, Jan

    2008-01-01

    Galaxy Zoo is the first study of nearby galaxies that contains reliable information about the spiral sense of rotation of galaxy arms for a sizeable number of galaxies. We measure the correlation function of spin chirality (the sense in which galaxies appear to be spinning) of face-on spiral galaxies in angular, real and projected spaces. Our results indicate a hint of positive correlation at separations less than ~0.5 Mpc at a statistical significance of 2-3 sigma. This is the first experimental evidence for chiral correlation of spins. Within tidal torque theory it indicates that the inertia tensors of nearby galaxies are correlated. This is complementary to the studies of nearby spin axis correlations that probe the correlations of the tidal field. Theoretical interpretation is made difficult by the small distances at which the correlations are detected, implying that substructure might play a significant role, and our necessary selection of face-on spiral galaxies, rather than a general volume-limited sam...

  5. Spin Transport by Collective Spin Excitations

    Science.gov (United States)

    Hammel, P. Chris

    We report studies of angular momentum transport in insulating materials. Our measurements reveal efficient spin pumping from high wavevector k spin waves in thin film Y3Fe5O12 (YIG): spin pumping is independent of wavevector up to k ~ 20 μm-1. Optical detection of YIG FMR by NV centers in diamond reveals a role for spin waves in this insulator-to-insulator spin transfer process. Spin transport is typically suppressed by insulating barriers, but we find that fluctuating antiferromagnetic correlations enable efficient spin transport at nm-scale thicknesses in insulating antiferromagnets, even in the absence of long-range order, and that the spin decay length increases with the strength of the antiferromagnetic correlations. This research is supported by the U.S. DOE through Grants DE-FG02-03ER46054 and DE-SC0001304, by the NSF MRSEC program through Grant No. 1420451 and by the Army Research Office through Grant W911NF0910147.

  6. Electrical manipulation of a ferromagnet by an antiferromagnet

    Science.gov (United States)

    Tshitoyan, V.; Ciccarelli, C.; Mihai, A. P.; Ali, M.; Irvine, A. C.; Moore, T. A.; Jungwirth, T.; Ferguson, A. J.

    Several recent studies of antiferromagnetic (AFM) spintronics have focused on transmission and detection of spin-currents in AFMs. Efficient spin transmission through AFMs was inferred from experiments in FM/AFM/NM (normal metal) structures. Measurements in FM/AFM bilayers have demonstrated that a metallic AFM can also act as an efficient ISHE detector of the spin-current, with spin-Hall angles comparable to heavy NMs. Here we demonstrate that an antiferromagnet can be employed for a highly efficient electrical manipulation of a ferromagnet. We use an all-electrical excitation and detection technique of ferromagnetic resonance in a NiFe/IrMn bilayer. We observe antidamping-like spin torque acting on the NiFe generated by the in-plane current driven through the IrMn antiferromagnet. A large enhancement of the torque, characterized by an effective spin-Hall angle exceeding most heavy transition metals, correlates with the presence of the exchange-bias field at the NiFe/IrMn interface. It highlights that, in addition to strong spin-orbit coupling, the AFM order in IrMn governs the observed phenomenon.

  7. Quantum dust magnetosonic waves with spin and exchange correlation effects

    Energy Technology Data Exchange (ETDEWEB)

    Maroof, R.; Qamar, A. [Department of Physics, University of Peshawar, Peshawar 25000 (Pakistan); Mushtaq, A. [Department of Physics, Abdul Wali Khan University, Mardan 23200 (Pakistan); National Center for Physics, Shahdra Valley Road, Islamabad 44000 (Pakistan)

    2016-01-15

    Dust magnetosonic waves are studied in degenerate dusty plasmas with spin and exchange correlation effects. Using the fluid equations of magnetoplasma with quantum corrections due to the Bohm potential, temperature degeneracy, spin magnetization energy, and exchange correlation, a generalized dispersion relation is derived. Spin effects are incorporated via spin force and macroscopic spin magnetization current. The exchange-correlation potentials are used, based on the adiabatic local-density approximation, and can be described as a function of the electron density. For three different values of angle, the dispersion relation is reduced to three different modes under the low frequency magnetohydrodynamic assumptions. It is found that the effects of quantum corrections in the presence of dust concentration significantly modify the dispersive properties of these modes. The results are useful for understanding numerous collective phenomena in quantum plasmas, such as those in compact astrophysical objects (e.g., the cores of white dwarf stars and giant planets) and in plasma-assisted nanotechnology (e.g., quantum diodes, quantum free-electron lasers, etc.)

  8. Role of correlations on spin-polarized neutron matter

    CERN Document Server

    Vidana, Isaac; Durant, Victoria

    2016-01-01

    Using the Hellmann--Feynman theorem we analyze the contribution of the different terms of the nucleon-nucleon interaction to the spin symmetry energy of neutron matter. The analysis is performed within the microscopic Brueckner--Hartree--Fock approach using the Argonne V18 realistic potential plus the Urbana IX three-body force. The main contribution to the spin-symmetry energy of neutron matter comes from the S=0 channel, acting only in the non-polarized neutron matter, in particular the $^1S_0$ and the $^1D_2$ partial waves. The importance of correlations in spin-polarized neutron matter is estimated by evaluating the kinetic energy difference between the correlated system and the underlying Fermi sea.

  9. Coherent and correlated spin transport in nanoscale superconductors

    Energy Technology Data Exchange (ETDEWEB)

    Morten, Jan Petter

    2008-03-15

    the system varies from e.g. ballistic conductors or tunnel barriers. In the tunneling case, we calculate the magnetization-dependent full counting statistics, which determines all noise properties including the cross-correlations that can resolve the contributions due to crossed Andreev reflection and direct electron transport. We evaluate the magnetization-dependent two-particle probability that the constituents of spin-entangled pairs from crossed Andreev reflection flow into different ferromagnetic contacts. This probability implies violation of a Bell inequality, and determines the performance of a superconductor-ferromagnet entangler. (author). 105 refs., 13 figs

  10. NMR on the antiferromagnetic S=1/2 Heisenberg spin chain Sr{sub 2}CuO{sub 3} under the impact of Ni impurities

    Energy Technology Data Exchange (ETDEWEB)

    Utz, Yannic; Hammerath, Franziska; Nishimoto, Satoshi; Drechsler, Stefan-Ludwig; Hess, Christian; Buechner, Bernd; Grafe, Hans-Joachim [IFW Dresden (Germany); Beesetty, Neela Sekhar; Saint-Martin, Romuald; Revcolevschi, Alexandre [SP2M-ICMMO UMR-CNRS, Universite Paris-Sud (France)

    2015-07-01

    We present {sup 63}Cu NMR measurements on single crystals of Sr{sub 2}CuO{sub 3} doped with different amounts of nickel and compare them to numerical DMRG results. The parent compound contains copper-oxygen chains with S=1/2 on the copper site coupled by a large antiferromagnetic exchange coupling J ∼ 2000 K and is known to be a good realization of the 1D Heisenberg model. The measurements show that replacing only a few of the S=1/2 Cu ions with S=1 Ni has a major impact on the magnetic properties of the spin chain system. An unusual line broadening in the low temperature NMR spectra reveals the existence of an impurity-induced local alternating magnetization (LAM), and exponentially decaying spin-lattice relaxation rates T{sup -1}{sub 1} towards low temperatures indicate the opening of a spin gap similar to Ca-doped Sr{sub 2}CuO{sub 3}. While the T{sup -1}{sub 1} measurements could be explained by pure chain segmentation, as expected for a S=0 impurity, the spectra can only be understood by taking the nickel.

  11. Reentrant phenomenon and inverse magnetocaloric effect in a generalized spin-(1/2,  s) Fisher's super-exchange antiferromagnet.

    Science.gov (United States)

    Gálisová, Lucia

    2016-11-30

    The thermodynamic and magnetocaloric properties of a generalized spin-(1/2,  s) Fisher's super-exchange antiferromagnet are investigated precisely by using the decoration-iteration mapping transformation. Besides the critical temperature, sublattice magnetization, total magnetization, entropy and specific heat, the isothermal entropy change and adiabatic temperature change are also rigorously calculated in order to examine the cooling efficiency of the model in the vicinity of the first- and second-order phase transitions. It is shown that an enhanced inverse magnetocaloric effect occurs around the temperature interval [Formula: see text] for any magnetic-field change [Formula: see text]. The most pronounced inverse magnetocaloric effect can be found nearby the critical field, which corresponds to the zero-temperature phase transition from the long-range ordered ground state to the paramagnetic one. The observed phenomenon increases with an increasing value of decorating spins. Furthermore, sufficiently high values of decorating spins have also been linked to the possibility of observing reentrant phase transitions at finite temperatures.

  12. Numerical evidence for a chiral spin liquid in the XXZ antiferromagnetic Heisenberg model on the kagome lattice at m =2/3 magnetization

    Science.gov (United States)

    Kumar, Krishna; Changlani, Hitesh J.; Clark, Bryan K.; Fradkin, Eduardo

    2016-10-01

    We perform an exact-diagonalization study of the spin-1/2 XXZ Heisenberg antiferromagnet on the kagome lattice at finite magnetization m =2/3 with an emphasis on the X Y point (Jz=0 ) and in the presence of a small chiral term. Recent analytic work by Kumar et al. [K. Kumar, K. Sun, and E. Fradkin, Phys. Rev. B 90, 174409 (2014), 10.1103/PhysRevB.90.174409] on the same model, using a newly developed flux attachment transformation, predicts a plateau at this value of the magnetization described by a chiral spin liquid (CSL) with a spin Hall conductance of σx y=1/2 . Such a state is topological in nature, has a ground-state degeneracy, and exhibits fractional excitations. We analyze the degeneracy structure in the low-energy manifold, identify the candidate topological states, and use them to compute the modular matrices and Chern numbers, all of which strongly agree with expected theoretical behavior for the σx y=1/2 CSL. In the limit of zero chirality, we find on most (not all) clusters that the topological invariants are still those of a CSL.

  13. Quantum phase transition, universality, and scaling behaviors in the spin-1/2 Heisenberg model with ferromagnetic and antiferromagnetic competing interactions on a honeycomb lattice.

    Science.gov (United States)

    Huang, Yi-Zhen; Xi, Bin; Chen, Xi; Li, Wei; Wang, Zheng-Chuan; Su, Gang

    2016-06-01

    The quantum phase transition, scaling behaviors, and thermodynamics in the spin-1/2 quantum Heisenberg model with antiferromagnetic coupling J>0 in the armchair direction and ferromagnetic interaction J^{'}Heisenberg O(3) universality. A zero magnetization plateau is observed in the dimerized phase, whose width decreases with increasing α. A phase diagram in the coupling ratio α-magnetic field h plane is obtained, where four phases, including dimerized, stripe, canted stripe, and polarized, are identified. It is also unveiled that the temperature dependence of the specific heat C(T) for different α's intersects precisely at one point, similar to that of liquid ^{3}He under different pressures and several magnetic compounds under various magnetic fields. The scaling behaviors of Q_{2}, ρ, and C(T) are carefully analyzed. The susceptibility is compared with the experimental data to give the magnetic parameters of both compounds.

  14. Magnetic Excitations and Electronic Interactions in Sr2 CuTeO6 : A Spin-1 /2 Square Lattice Heisenberg Antiferromagnet

    Science.gov (United States)

    Babkevich, P.; Katukuri, Vamshi M.; Fâk, B.; Rols, S.; Fennell, T.; Pajić, D.; Tanaka, H.; Pardini, T.; Singh, R. R. P.; Mitrushchenkov, A.; Yazyev, O. V.; Rønnow, H. M.

    2016-12-01

    Sr2 CuTeO6 presents an opportunity for exploring low-dimensional magnetism on a square lattice of S =1 /2 Cu2 + ions. We employ ab initio multireference configuration interaction calculations to unravel the Cu2 + electronic structure and to evaluate exchange interactions in Sr2 CuTeO6 . The latter results are validated by inelastic neutron scattering using linear spin-wave theory and series-expansion corrections for quantum effects to extract true coupling parameters. Using this methodology, which is quite general, we demonstrate that Sr2 CuTeO6 is an almost ideal realization of a nearest-neighbor Heisenberg antiferromagnet but with relatively weak coupling of 7.18(5) meV.

  15. Large-scale numerical investigations of the antiferromagnetic Heisenberg icosidodecahedron

    Energy Technology Data Exchange (ETDEWEB)

    Ummethum, Joerg [Department of Physics, Bielefeld University, P.O. Box 100131, D-33501 Bielefeld (Germany); Schnack, Juergen, E-mail: jschnack@uni-bielefeld.de [Department of Physics, Bielefeld University, P.O. Box 100131, D-33501 Bielefeld (Germany); Laeuchli, Andreas M. [Inst. f. Theoretische Physik, Innsbruck University, Technikerstr. 25, 6020 Innsbruck (Austria)

    2013-02-15

    We present up to date investigations of the antiferromagnetic Heisenberg icosidodecahedron by means of the density matrix renormalization group method. We compare our results with modern correlator product state as well as Lanczos calculations. - Highlights: Black-Right-Pointing-Pointer Results of unprecedented accuracy for energies and correlation functions of a frustrated spin system. Black-Right-Pointing-Pointer Relevance for a large set of magnetic molecules. Black-Right-Pointing-Pointer Demonstration of accuracy of DDMRG.

  16. Electron Spin Pairing in High-Tc Superconductors

    Institute of Scientific and Technical Information of China (English)

    郭卫; 韩汝珊

    2001-01-01

    An electron pairing theory based on effective electron spin coupling mediated by antiferromagnetically correlated local moments is presented to account for high-Tc phenomena. We show that Kondo scattering and the suppression of the antiferromagnetic superexchange between Cu2+ moments lead to local triplet pairing, the mechanism underlying high-Tc superconductivity.

  17. Spin gap and antiferromagnetic correlations in the kondo insulator CeNiSn

    DEFF Research Database (Denmark)

    Mason, T.E.; Aeppli, G.; Ramirez, A.P.

    1992-01-01

    Neutron scattering measurements show that the crossover (at T less than or similar to 10 K) from metallic heavy-fermion to semiconducting behavior coincides with the formation of a gap in the magnetic excitation spectrum of CeNiSn. In contrast to the simple band picture of an insulator, the gap...

  18. Magnetization processes and transitions between two antiferromagnetic spin configurations in single-crystalline MnSn2

    Science.gov (United States)

    Duan, T. F.; Ren, W. J.; Liu, W.; Zhang, Z. D.

    2016-08-01

    The magnetic structure of MnSn2 and magnetic phase transitions in this compound have been investigated by magnetic measurements on single crystals. The results show that two antiferromagnetic (AFM) states exist below 325 K and that a transition between these two phases occurs at 74 K. Applying a magnetic field (H) has great influence on the transition temperature. An anomalous magnetization process at low fields occurs when the magnetic field applied along the [110] direction, which is ascribed to the contribution of the basal anisotropy. Based on the data for the magnetization processes and the phase transition of the present single crystal, the H-T phase diagram has been established.

  19. Antiferromagnetic correlations in icosahedral R-Mg-Zn quasicrystals (R rare earth)

    Energy Technology Data Exchange (ETDEWEB)

    Charrier, B.; Schmitt, D. [Centre National de la Recherche Scientifique (CNRS), 38 - Grenoble (France); Ouladdiaf, B. [Institut Max von Laue - Paul Langevin (ILL), 38 - Grenoble (France)

    1997-04-01

    Powder neutron-diffraction experiments performed on R-Mg-Zn quasicrystals have shown for the first time the existence of magnetic ordering of the rare earth in these systems at low temperature (T{sub c} {<=} 6.5 K depending on the rare earth). Both narrow and broad magnetic diffraction peaks have been observed showing the presence of two different scales of magnetic correlations. (author). 3 refs.

  20. Effects of coexisting spin disorder and antiferromagnetism on the magnetic behavior of nanostructured (Fe{sub 79}Mn{sub 21}){sub 1−x}Cu{sub x} alloys

    Energy Technology Data Exchange (ETDEWEB)

    Mizrahi, M., E-mail: mizrahi@fisica.unlp.edu.ar, E-mail: cabrera@fisica.unlp.edu.ar [INIFTA-CCT- La Plata-CONICET and Departamento de Física, Facultad de Ciencias Exactas, C. C. 67, Universidad Nacional de La Plata, 1900 La Plata (Argentina); Cabrera, A. F., E-mail: mizrahi@fisica.unlp.edu.ar, E-mail: cabrera@fisica.unlp.edu.ar; Desimoni, J. [IFLP-CCT-La Plata-CONICET and Departamento de Física, Facultad de Ciencias Exactas C.C. 67, Universidad Nacional de La Plata, 1900 La Plata (Argentina); Stewart, S. J. [IFLP-CCT-La Plata-CONICET and Departamento de Física, Facultad de Ciencias Exactas C.C. 67, Universidad Nacional de La Plata, 1900 La Plata (Argentina); Instituto Ciencias de la Salud, Universidad Nacional Arturo Jauretche, Av. Calchaquí No. 6200, Florencio Varela (Argentina)

    2014-06-07

    We report a magnetic study on nanostructured (Fe{sub 79}Mn{sub 21}){sub 1−x}Cu{sub x} (0.00 ≤ x ≤ 0.30) alloys using static magnetic measurements. The alloys are mainly composed by an antiferromagnetic fcc phase and a disordered region that displays a spin-glass-like behavior. The interplay between the antiferromagnetic and magnetically disordered phases establishes an exchange anisotropy that gives rise to a loop shift at temperatures below the freezing temperature of moments belonging to the disordered region. The loop shift is more noticeable as the Cu content increases, which also enhances the spin-glass-like features. Further, in the x = 0.30 alloy the alignment imposed by applied magnetic fields higher than 4 kOe prevail over the configuration determined by the frustration mechanism that characterizes the spin glass-like phase.

  1. Frustrated spin correlations in diluted spin ice Ho2-xLaxTi2O7

    Energy Technology Data Exchange (ETDEWEB)

    Ehlers, Georg; Ehlers, G.; Mamontov, E.; Zamponi, M.; Faraone, A.; Qiu, Y.; Cornelius, A.L.; Booth, C.H.; Kam, K.C.; Le Toquin, R.; Cheetham, A.K.; Gardner, J.S.

    2008-04-30

    We have studied the evolution of the structural properties as well as the static and dynamic spin correlations of spin ice Ho2Ti2O7, where Ho was partially replaced by non-magnetic La. The crystal structure of diluted samples Ho2-xLaxTi2O7 was characterized by x-ray and neutron diffraction and by Ho L-III-edge and Ti K-edge extended x-ray absorption fine structure (EXAFS) measurements. It is found that the pyrochlore structure remains intact until about x = 0.3, but a systematic increase in local disorder with increasing La concentration is observed in the EXAFS data, especially from the Ti K edge.Quasi-elastic neutron scattering and ac susceptibility measurements show that, in x<= 0.4 samples at temperatures above macroscopic freezing, the spin -spin correlations are short ranged and dynamic in nature. The main difference with pure spin ice in the dynamics is the appearance of a second, faster, relaxation process.

  2. Mixed-state quantum transport in correlated spin networks

    CERN Document Server

    Ajoy, Ashok; 10.1103/PhysRevA.85.042305

    2012-01-01

    Quantum spin networks can be used to transport information between separated registers in a quantum information processor. To find a practical implementation, the strict requirements of ideal models for perfect state transfer need to be relaxed, allowing for complex coupling topologies and general initial states. Here we analyze transport in complex quantum spin networks in the maximally mixed state and derive explicit conditions that should be satisfied by propagators for perfect state transport. Using a description of the transport process as a quantum walk over the network, we show that it is necessary to phase correlate the transport processes occurring along all the possible paths in the network. We provide a Hamiltonian that achieves this correlation, and use it in a constructive method to derive engineered couplings for perfect transport in complicated network topologies.

  3. Pressure effect on the competition between ferromagnetic and antiferromagnetic spin fluctuations in TmTe investigated by 125Te-NMR

    Science.gov (United States)

    Yamamoto, A.; Wada, S.; Matsumura, T.

    2007-03-01

    To elucidate from a microscopic point of view the initial evolution of spin fluctuations in TmTe from the semiconducting state at ambient pressure with an antiferroquadrupole ordering (TQ=1.8 K) to the intermediate-valence metallic state at high pressures P⩾2 GPa with a ferromagnetic (FM) ordering (TC≃14 K), we have carried out 125Te-NMR study at pressures P=0 and 0.9 GPa. The spin-lattice relaxation rate measurements revealed a pronounced increase of the staggered susceptibility below T*≃14 K, in addition to the Curie-Weiss-type increase of the uniform susceptibility. Below ˜T*, a wipe-out decrease of the NMR intensity and the finding of an unconventional NMR signal around ˜10 MHz that is insensitive to applied field lead to the conclusion that a field-induced short-range FM ordering caused by the competition of FM and antiferromagnetic fluctuations takes place. Pressure of 0.9 GPa hardly affects the anomalous NMR behaviors below ˜T*, leading to speculate that the short-range FM ordering in the semiconducting state shares the origin with the long-range FM ordering at ≃14 K in the high-pressure metallic state.

  4. Approximate Counting via Correlation Decay in Spin Systems

    CERN Document Server

    Li, Liang; Yin, Yitong

    2011-01-01

    We give the first deterministic fully polynomial-time approximation scheme (FPTAS) for computing the partition function of a two-state spin system on an arbitrary graph, when the parameters of the system satisfy the uniqueness condition on infinite regular trees. This condition is of physical significance and is believed to be the right boundary between approximable and inapproximable. The FPTAS is based on the correlation decay technique introduced by Bandyopadhyay and Gamarnik [SODA 06] and Weitz [STOC 06]. The classic correlation decay is defined with respect to graph distance. Although this definition has natural physical meanings, it does not directly support an FPTAS for systems on arbitrary graphs, because for graphs with unbounded degrees, the local computation that provides a desirable precision by correlation decay may take super-polynomial time. We introduce a notion of \\concept{computationally efficient correlation decay}, in which the correlation decay is measured in a refined metric instead of g...

  5. First example of a high-level correlated calculation of the indirect spin-spin coupling constants involving tellurium

    DEFF Research Database (Denmark)

    Rusakov, Yury Yu; Krivdin, Leonid B.; Østerstrøm, Freja From;

    2013-01-01

    This paper documents a very first example of a high-level correlated calculation of spin-spin coupling constants involving tellurium taking into account relativistic effects, vibrational corrections and solvent effects for the medium sized organotellurium molecules. The 125Te-1H spin-spin coupling...... of spin-spin coupling constants involving tellurium, was developed. The SOPPA methods show much better performance as compared to 15 those of DFT, if relativistic effects calculated within the ZORA scheme are taken into account. Vibrational and solvent corrections are next to negligible, while...

  6. Angular dependence of dipole-dipole-Curie-spin cross-correlation effects in high-spin and low-spin paramagnetic myoglobin.

    Science.gov (United States)

    Pintacuda, Guido; Hohenthanner, Karin; Otting, Gottfried; Müller, Norbert

    2003-10-01

    The (15)N-HSQC spectra of low-spin cyano-met-myoglobin and high-spin fluoro-met-myoglobin were assigned and dipole-dipole-Curie-spin cross-correlated relaxation rates measured. These cross-correlation rates originating from the dipolar (1)H-(15)N interaction and the dipolar interaction between the (1)H and the Curie spin of the paramagnetic center contain long-range angular information about the orientation of the (1)H-(15)N bond with respect to the iron-(1)H vector, with information measurable up to 11 A from the metal for the low-spin complex, and between 10 to 25 A for the high-spin complex. Comparison of the experimental data with predictions from crystal structure data showed that the anisotropy of the magnetic susceptibility tensor in low spin cyano-met-myoglobin significantly influences the cross-correlated dipole-dipole-Curie-spin relaxation rates.

  7. Onset of antiferromagnetism in heavy-fermion metals

    Science.gov (United States)

    Schroder; Aeppli; Coldea; Adams; Stockert; v. Lohneysen H; Bucher; Ramazashvili; Coleman

    2000-09-21

    There are two main theoretical descriptions of antiferromagnets. The first arises from atomic physics, which predicts that atoms with unpaired electrons develop magnetic moments. In a solid, the coupling between moments on nearby ions then yields antiferromagnetic order at low temperatures. The second description, based on the physics of electron fluids or 'Fermi liquids' states that Coulomb interactions can drive the fluid to adopt a more stable configuration by developing a spin density wave. It is at present unknown which view is appropriate at a 'quantum critical point' where the antiferromagnetic transition temperature vanishes. Here we report neutron scattering and bulk magnetometry measurements of the metal CeCu(6-x)Au(x), which allow us to discriminate between the two models. We find evidence for an atomically local contribution to the magnetic correlations which develops at the critical gold concentration (x(c) = 0.1), corresponding to a magnetic ordering temperature of zero. This contribution implies that a Fermi-liquid-destroying spin-localizing transition, unanticipated from the spin density wave description, coincides with the antiferromagnetic quantum critical point.

  8. Electrical manipulation of ferromagnetic NiFe by antiferromagnetic IrMn

    Science.gov (United States)

    Tshitoyan, V.; Ciccarelli, C.; Mihai, A. P.; Ali, M.; Irvine, A. C.; Moore, T. A.; Jungwirth, T.; Ferguson, A. J.

    2015-12-01

    We demonstrate that an antiferromagnet can be employed for a highly efficient electrical manipulation of a ferromagnet. In our study, we use an electrical detection technique of the ferromagnetic resonance driven by an in-plane ac current in a NiFe/IrMn bilayer. At room temperature, we observe antidampinglike spin torque acting on the NiFe ferromagnet, generated by an in-plane current driven through the IrMn antiferromagnet. A large enhancement of the torque, characterized by an effective spin-Hall angle exceeding most heavy transition metals, correlates with the presence of the exchange-bias field at the NiFe/IrMn interface. It highlights that, in addition to the strong spin-orbit coupling, the antiferromagnetic order in IrMn governs the observed phenomenon.

  9. Quantum correlations and coherence in spin-1 Heisenberg chains

    Science.gov (United States)

    Malvezzi, A. L.; Karpat, G.; ćakmak, B.; Fanchini, F. F.; Debarba, T.; Vianna, R. O.

    2016-05-01

    We explore quantum and classical correlations along with coherence in the ground states of spin-1 Heisenberg chains, namely the one-dimensional XXZ model and the one-dimensional bilinear biquadratic model, with the techniques of density matrix renormalization group theory. Exploiting the tools of quantum information theory, that is, by studying quantum discord, quantum mutual information, and three recently introduced coherence measures in the reduced density matrix of two nearest neighbor spins in the bulk, we investigate the quantum phase transitions and special symmetry points in these models. We point out the relative strengths and weaknesses of correlation and coherence measures as figures of merit to witness the quantum phase transitions and symmetry points in the considered spin-1 Heisenberg chains. In particular, we demonstrate that, as none of the studied measures can detect the infinite-order Kosterlitz-Thouless transition in the XXZ model, they appear to be able to signal the existence of the same type of transition in the biliear biquadratic model. However, we argue that what is actually detected by the measures here is the SU(3) symmetry point of the model rather than the infinite-order quantum phase transition. Moreover, we show in the XXZ model that examining even single site coherence can be sufficient to spotlight the second-order phase transition and the SU(2) symmetry point.

  10. Unveiling the origin of the basal-plane antiferromagnetism in the spin-orbit Mott insulator Ba2IrO4: a density functional and model Hamiltonian study

    Science.gov (United States)

    Hou, Y. S.; Xiang, H. J.; Gong, X. G.

    2016-04-01

    Based on the density functional theory and model Hamiltonian, we studied the basal-plane antiferromagnetism in the spin-orbit Mott insulator Ba2IrO4. By comparing the magnetic properties of the bulk Ba2IrO4 with those of the single-layer Ba2IrO4, we demonstrate unambiguously that the basal-plane antiferromagnetism is caused by the intralyer magnetic interactions rather than by the previously proposed interlayer ones. Aiming at revealing the origin of the basal-plane antiferromagnetism, we add the single ion anisotropy and pseudo-quadrupole interactions into the general bilinear pseudo-spin Hamiltonian. The obtained magnetic interaction parameters indicate that the single ion anisotropy and pseudo-quadrupole interactions are unexpectedly strong. Systematical Monte Carlo simulations demonstrate that the basal-plane antiferromagnetism is caused by isotropic Heisenberg, bond-dependent Kitaev and pseudo-quadrupole interactions. On the basis of this study the single ion anisotropy and pseudo-quadrupole interactions could play a role in explaining magnetic interactions in other iridates.

  11. Strongly correlated flat-band systems: The route from Heisenberg spins to Hubbard electrons

    Science.gov (United States)

    Derzhko, Oleg; Richter, Johannes; Maksymenko, Mykola

    2015-05-01

    On a large class of lattices (such as the sawtooth chain, the kagome and the pyrochlore lattices), the quantum Heisenberg and the repulsive Hubbard models may host a completely dispersionless (flat) energy band in the single-particle spectrum. The flat-band states can be viewed as completely localized within a finite volume (trap) of the lattice and allow for construction of many-particle states, roughly speaking, by occupying the traps with particles. If the flat-band happens to be the lowest-energy one, the manifold of such many-body states will often determine the ground-state and low-temperature physics of the models at hand even in the presence of strong interactions. The localized nature of these many-body states makes possible the mapping of this subset of eigenstates onto a corresponding classical hard-core system. As a result, the ground-state and low-temperature properties of the strongly correlated flat-band systems can be analyzed in detail using concepts and tools of classical statistical mechanics (e.g., classical lattice-gas approach or percolation approach), in contrast to more challenging quantum many-body techniques usually necessary to examine strongly correlated quantum systems. In this review, we recapitulate the basic features of the flat-band spin systems and briefly summarize earlier studies in the field. The main emphasis is made on recent developments which include results for both spin and electron flat-band models. In particular, for flat-band spin systems, we highlight field-driven phase transitions for frustrated quantum Heisenberg antiferromagnets at low temperatures, chiral flat-band states, as well as the effect of a slight dispersion of a previously strictly flat-band due to nonideal lattice geometry. For electronic systems, we discuss the universal low-temperature behavior of several flat-band Hubbard models, the emergence of ground-state ferromagnetism in the square-lattice Tasaki-Hubbard model and the related Pauli-correlated

  12. Thermoinduced magnetization in nanoparticles of antiferromagnetic materials

    DEFF Research Database (Denmark)

    Mørup, Steen; Frandsen, Cathrine

    2004-01-01

    We show that there is a thermoinduced contribution to the magnetic moment of nanoparticles of antiferromagnetic materials. It arises from thermal excitations of the uniform spin-precession mode, and it has the unusual property that its magnitude increases with increasing temperature. This has...... the consequence that antiferromagnetism is nonexistent in nanoparticles at finite temperatures and it explains magnetic anomalies, which recently have been reported in a number of studies of nanoparticles of antiferromagnetic materials....

  13. Correlation between peak and median blocking temperatures by magnetization measurement on isolated ferromagnetic and antiferromagnetic particle systems

    DEFF Research Database (Denmark)

    Jiang, Jianzhong; Mørup, Steen

    1997-01-01

    The influence of the particle size distribution on the ratio of the peak temperature, T-peak, to the blocking temperature, T-Bm, in zero field cooled (ZFD) magnetization curves has studied for both ferromagnetic and antiferromagnetic particle systems. In both systems the ratio beta=T-peak/T-Bm does...

  14. Molecular spin on surface: From strong correlation to dispersion interactions

    Science.gov (United States)

    Zhang, Yachao

    2016-09-01

    A reliable prediction of magnetic properties of surface-supported molecules containing 3d/4f spin carriers has challenged the electronic structure theory for decades. Here we tackle this problem with Hubbard-U corrected van der Waals density functional (vdW-DF), incorporating strong correlation effects of the localized electrons and dispersion interactions involved in the molecule-surface binding. By fitting the spin state energetics of a series of Fe(ii) compounds with varying ligand field strength, we find that the optimal U value for vdW-DF is much smaller than that for the local density approximation (LDA) while quite similar to that for the generalized gradient approximation (GGA). We show that although vdW-DF+U overestimates largely the metal-ligand bond distance, the predicted adiabatic high-spin-low-spin energy splitting ΔEHL is only slightly changed with respect to that obtained using the LDA+U geometries consistent with experiment. Then we use Cu(111)-supported metallocene (M(C5H5)2, M = Fe, and Co) as a prototype example to explore the effects of the molecule-surface interactions. We show that the non-local dispersion interactions, poorly described by LDA and GGA while reasonably captured by vdW-DF, are critical for reproducing ΔEHL at large molecule-surface distances. Besides, we find that ΔEHL is decreased by the molecule-metal contact, which is shown to weaken the local ligand field around the magnetic center.

  15. Numerical study of magnetization plateaus in the spin-1/2 Heisenberg antiferromagnet on the checkerboard lattice

    Science.gov (United States)

    Capponi, Sylvain

    2017-01-01

    We present numerical evidence that the spin-1/2 Heisenberg model on the two-dimensional checkerboard lattice exhibits several magnetization plateaus for m =0 , 1 /4 , 1 /2 , and 3 /4 , where m is the magnetization normalized by its saturation value. These incompressible states correspond to somewhat similar valence-bond crystal phases that break lattice symmetries, though they are different from the already established plaquette phase for m =0 . Our results are based on exact diagonalization as well as density-matrix renormalization-group large-scale simulations and interpreted in terms of simple parameter-free trial wave functions.

  16. Quantum Disordered State without Frustration in the Double Layer Heisenberg Antiferromagnet —Dimer Expansion and Projector Monte Carlo Study—

    Science.gov (United States)

    Hida, Kazuo

    1992-03-01

    The quantum disordered state (QDOS) of the spin 1/2 double layer square lattice Heisenberg antiferromagnet is studied. Using the dimer expansion from the limit of the large interlayer coupling J', the staggered susceptibility χ, the antiferromagnetic structure factor Sπ and the antiferromagnetic correlation length ξ are calculated up to the 6-th order in the intralayer coupling J. The ratio analysis shows that the QDOS becomes unstable against the Néel ordering at J'/J≃2.56. The critical exponents are not inconsistent with the universality class of the 3-dimensional classical Heisenberg model, suggesting that our QDOS corresponds to that expected in the 2-dimensional square lattice Heisenberg antiferromagnet with unphysically small spin (<0.276). The results of the projector Monte Carlo simulation also confirms the dimer expansion results.

  17. Gapless spin liquid ground state in the S = 1/2 vanadium oxyfluoride kagome antiferromagnet [NH4]2[C7H14N][V7O6F18].

    Science.gov (United States)

    Clark, L; Orain, J C; Bert, F; De Vries, M A; Aidoudi, F H; Morris, R E; Lightfoot, P; Lord, J S; Telling, M T F; Bonville, P; Attfield, J P; Mendels, P; Harrison, A

    2013-05-17

    The vanadium oxyfluoride [NH(4)](2)[C(7)H(14)N][V(7)O(6)F(18)] (DQVOF) is a geometrically frustrated magnetic bilayer material. The structure consists of S = 1/2 kagome planes of V(4+) d(1) ions with S = 1 V(3+) d(2) ions located between the kagome layers. Muon spin relaxation measurements demonstrate the absence of spin freezing down to 40 mK despite an energy scale of 60 K for antiferromagnetic exchange interactions. From magnetization and heat capacity measurements we conclude that the S = 1 spins of the interplane V(3+) ions are weakly coupled to the kagome layers, such that DQVOF can be viewed as an experimental model for S = 1/2 kagome physics, and that it displays a gapless spin liquid ground state.

  18. Dynamical Structure Factors of quasi-one-dimensional antiferromagnets

    Science.gov (United States)

    Hagemans, Rob; Caux, Jean-Sébastien; Maillet, Jean Michel

    2007-03-01

    For a long time it has been impossible to accurately calculate the dynamical structure factors (spin-spin correlators as a function of momentum and energy) of quasi-one-dimensional antiferromagnets. For integrable Heisenberg chains, the recently developed ABACUS method (a first-principles computational approach based on the Bethe Ansatz) now yields highly accurate (over 99% of the sum rule) results for the DSF for finite chains, allowing for a very precise description of neutron-scattering data over the full momentum and energy range. We show remarkable agreement between results obtained with ABACUS and experiment.

  19. Spin valves based on Mn{sub 75}Ir{sub 25} antiferromagnet with controllable functional parameters

    Energy Technology Data Exchange (ETDEWEB)

    Milyaev, M. A., E-mail: milyaev@imp.uran.ru; Naumova, L. I.; Kamenskii, I. Yu.; Ustinov, V. V. [Russian Academy of Sciences, Institute of Metal Physics, Ural Branch (Russian Federation)

    2015-12-15

    Using the example of spin valves of the Ta(50 Å)/Ni{sub 80}Fe{sub 20}(30 Å)/Co{sub 90}Fe{sub 10}(15 Å)/Cu(28 Å)/Co{sub 90}Fe{sub 10}(20 Å)/Mn{sub 75}Ir{sub 25}(50 Å)/Ta(20 Å) composition, factors controlling the hysteresis properties are studied for the case of macro- and microscopic sizes of an experimental sample. It is shown that a linear change in the magnetoresistance with small hysteresis while retaining the giant magnetoresistance effect at a level of 8% can be obtained in a micro-object (meander) using thermomagnetic treatment.

  20. Charge transport and magnetization profile at the interface between the correlated metal CaRuO3 and the antiferromagnetic insulator CaMnO3

    Energy Technology Data Exchange (ETDEWEB)

    Freeland, J. W. [Argonne National Laboratory (ANL); Chakhalian, J. [University of Arkansas; Boris, A. V. [Max-Planck-Institut fur Feskorperforschung, Stuttgart, Germany; Tonnerre, J.-M. [CNRS, France; Kavich, J. J. [University of Illinois, Chicago; Yordanov, P. [Max-Planck-Institut fur Feskorperforschung, Stuttgart, Germany; Grenier, S. [CNRS, Grenoble, France; Lee, Ho Nyung [ORNL; Keimer, Bernhard [Max-Planck-Institut fur Feskorperforschung, Stuttgart, Germany

    2010-01-01

    A combination of spectroscopic probes was used to develop a detailed experimental description of the transport and magnetic properties of superlattices composed of the paramagnetic metal CaRuO3 and the antiferromagnetic insulator CaMnO3. The charge carrier density and Ru valence state in the superlattices are not significantly different from those of bulk CaRuO3. The small charge transfer across the interface implied by these observations confirms predictions derived from density functional calculations. However, a ferromagnetic polarization due to canted Mn spins penetrates 3-4 unit cells into CaMnO3, far exceeding the corresponding predictions. The discrepancy may indicate the formation of magnetic polarons at the interface.

  1. Band structure of the heavily-electron-doped FeAs-based Ba(Fe,Co)2As2 superconductor suppresses antiferromagnetic correlations.

    Science.gov (United States)

    Sudayama, T; Wakisaka, Y; Takubo, K; Morinaga, R; Sato, T J; Arita, M; Namatame, H; Taniguchi, M; Mizokawa, T

    2010-04-30

    In the heavily-electron-doped regime of the Ba(Fe,Co)2As2 superconductor, three hole bands at the zone center are observed and two of them reach the Fermi level. The larger hole pocket at the zone center is apparently nested with the smaller electron pocket around the zone corner. However, the (pi,0) Fermi surface reconstruction reported for the hole-doped case is absent in the heavily-electron-doped case. This observation shows that the apparent Fermi surface nesting alone is not enough to enhance the antiferromagnetic correlation as well as the superconducting transition temperature.

  2. Dynamical correlation functions of the S=1/2 nearest-neighbor and Haldane-Shastry Heisenberg antiferromagnetic chains in zero and applied fields

    DEFF Research Database (Denmark)

    Lefmann, K.; Rischel, C.

    1996-01-01

    We present a numerical diagonalization study of two one-dimensional S=1/2 antiferromagnetic Heisenberg chains, having nearest-neighbor and Haldane-Shastry (1/r(2)) interactions, respectively. We have obtained the T=0 dynamical correlation function, S-alpha alpha(q,omega), for chains of length N=8......-28. We have studied S-zz(q,omega) for the Heisenberg chain in zero field, and from finite-size scaling we have obtained a limiting behavior that for large omega deviates from the conjecture proposed earlier by Muller ct al. For both chains we describe the behavior of S-zz(q,omega) and S...

  3. Evidence of an odd-parity hidden order in a spin-orbit coupled correlated iridate

    Science.gov (United States)

    Zhao, L.; Torchinsky, D. H.; Chu, H.; Ivanov, V.; Lifshitz, R.; Flint, R.; Qi, T.; Cao, G.; Hsieh, D.

    2016-01-01

    A rare combination of strong spin-orbit coupling and electron-electron correlations makes the iridate Mott insulator Sr2IrO4 a promising host for novel electronic phases of matter. The resemblance of its crystallographic, magnetic and electronic structures to La2CuO4, as well as the emergence on doping of a pseudogap region and a low-temperature d-wave gap, has particularly strengthened analogies to cuprate high-Tc superconductors. However, unlike the cuprate phase diagram, which features a plethora of broken symmetry phases in a pseudogap region that includes charge density wave, stripe, nematic and possibly intra-unit-cell loop-current orders, no broken symmetry phases proximate to the parent antiferromagnetic Mott insulating phase in Sr2IrO4 have been observed so far, making the comparison of iridate to cuprate phenomenology incomplete. Using optical second-harmonic generation, we report evidence of a hidden non-dipolar magnetic order in Sr2IrO4 that breaks both the spatial inversion and rotational symmetries of the underlying tetragonal lattice. Four distinct domain types corresponding to discrete 90°-rotated orientations of a pseudovector order parameter are identified using nonlinear optical microscopy, which is expected from an electronic phase that possesses the symmetries of a magneto-electric loop-current order. The onset temperature of this phase is monotonically suppressed with bulk hole doping, albeit much more weakly than the Néel temperature, revealing an extended region of the phase diagram with purely hidden order. Driving this hidden phase to its quantum critical point may be a path to realizing superconductivity in Sr2IrO4.

  4. Field-Induced Multiple Reentrant Quantum Phase Transitions in Randomly Dimerized Antiferromagnetic S=1/2 Heisenberg Chains

    Science.gov (United States)

    Hida, Kazuo

    2006-07-01

    The multiple reentrant quantum phase transitions in the S=1/2 antiferromagnetic Heisenberg chains with random bond alternation in the magnetic field are investigated by the density matrix renormalization group method combined with interchain mean field approximation. It is assumed that odd numbered bonds are antiferromagnetic with strength J and even numbered bonds can take the values JS and JW (JS > J > JW > 0) randomly with the probabilities p and 1- p, respectively. The pure version ( p=0 and 1) of this model has a spin gap but exhibits a field-induced antiferromagnetism in the presence of interchain coupling if Zeeman energy due to the magnetic field exceeds the spin gap. For 0 < p < 1, antiferromagnetism is induced by randomness at the small field region where the ground state is disordered due to the spin gap in the pure version. At the same time, this model exhibits randomness-induced plateaus at several values of magnetization. The antiferromagnetism is destroyed on the plateaus. As a consequence, we find a series of reentrant quantum phase transitions between transverse antiferromagnetic phases and disordered plateau phases with the increase of magnetic field for a moderate strength of interchain coupling. Above the main plateaus, the magnetization curve consists of a series of small plateaus and jumps between them. It is also found that antiferromagnetism is induced by infinitesimal interchain coupling at the jumps between the small plateaus. We conclude that this antiferromagnetism is supported by the mixing of low-lying excited states by the staggered interchain mean field even though the spin correlation function is short ranged in the ground state of each chain.

  5. Itinerant antiferromagnetism in the Mott compound V1.973O3

    Science.gov (United States)

    Bao, Wei; Broholm, C.; Honig, J. M.; Metcalf, P.; Trevino, S. F.

    1996-08-01

    The doping-induced metallic state of the Mott system V2-yO3 has spin-density-wave order for Tspin correlations in such a cation-deficient sample, V1.973O3, were measured with inelastic neutron scattering throughout the Brillouin zone for energies up to ~20kBTN and temperatures up to ~20TN. The dynamic spin-correlation function, S(q,ω), consists of a single ridge as a function of ħω centered at each antiferromagnetic Bragg point. The q, ω, and T dependence of magnetic fluctuations can be described by the self-consistent renormalization theory for weak itinerant antiferromagnets developed by Moriya, Hasegawa, and Nakayama. Thermodynamic properties below ~10TN are quantitatively accounted for by this theory in its simplest form with only four parameters, which are determined by our neutron-scattering experiment.

  6. Spin-noise correlations and spin-noise exchange driven by low-field spin-exchange collisions

    OpenAIRE

    Dellis, A. T.; Loulakis, M.; Kominis, I. K.

    2013-01-01

    The physics of spin exchange collisions have fueled several discoveries in fundamental physics and numerous applications in medical imaging and nuclear magnetic resonance. We here report on the experimental observation and theoretical justification of spin-noise exchange, the transfer of spin-noise from one atomic species to another. The signature of spin-noise exchange is an increase of the total spin-noise power at low magnetic fields, on the order of 1 mG, where the two-species spin-noise ...

  7. μ SR insight into the impurity problem in quantum kagome antiferromagnets

    Science.gov (United States)

    Gomilšek, M.; Klanjšek, M.; Pregelj, M.; Luetkens, H.; Li, Y.; Zhang, Q. M.; Zorko, A.

    2016-07-01

    Impurities, which are unavoidable in real materials, may play an important role in the magnetism of frustrated spin systems with a spin-liquid ground state. We address the impurity issue in quantum kagome antiferromagnets by investigating ZnCu3(OH) 6SO4 (Zn-brochantite) by means of muon spin spectroscopy. We show that muons dominantly couple to impurities, originating from Cu-Zn intersite disorder, and that the impurity spins are highly correlated with the kagome spins, allowing us to probe the host kagome physics via a Kondo-like effect. The low-temperature plateau in the impurity susceptibility suggests that the kagome spin-liquid ground state is gapless. The corresponding spin fluctuations exhibit an unconventional spectral density and a nontrivial field dependence.

  8. Determinant representations for correlation functions of spin-1/2 Heisenberg XXZ magnets

    CERN Document Server

    Essler, F H L; Izergin, A G; Korepin, V E

    1994-01-01

    We consider correlation functions of the spin-\\half XXX and XXZ Heisenberg chains in a magnetic field. Starting from the algebraic Bethe Ansatz we derive representations for various correlation functions in terms of determinants of Fredholm integral operators.

  9. Fisher-Hartwig conjecture and the correlators in XY spin chain

    Energy Technology Data Exchange (ETDEWEB)

    Ovchinnikov, A.A. [Institute for Nuclear Research, RAS, Moscow 117312 (Russian Federation)]. E-mail: ovch@ms2.inr.ac.ru

    2007-07-02

    We apply the theorems from the theory of Toeplitz determinants to calculate the asymptotics of the correlators in the XY spin chain in the transverse magnetic field. The asymptotics of the correlators for the XX spin chain in the magnetic field are obtained.

  10. Thermodynamics of strongly disordered spin ladders

    OpenAIRE

    Yusuf, Eddy; Yang, Kun

    2002-01-01

    We study antiferromagnetic two-leg spin-1/2 ladders with strong bond randomness, using the real space renormalization group method. We find the low-temperature spin susceptibility of the system follows non-universal power laws, and the ground state spin-spin correlation is short-ranged. Our results suggest that there is no phase transition when the bond randomness increases from zero; for strong enough randomness the system is in a Griffith region with divergent spin susceptibility and short-...

  11. Investigation of the Spin-glass Regime Between the Antiferromagnetic and Superconducting Phases in Fe1+ySexTe1−x

    Energy Technology Data Exchange (ETDEWEB)

    Katayama, N.; Wen, J.; Ji, S.; Louca, D.; Lee, S.-H.; Fujita, M.; Sato, T.J.; Wen, J.S.; Xu, Z.J.; Gu, G.D.; Xu, G.; Lin, Z.W.; Enoki, M.; Chang, S.; Yamada, K.; Tranquada, J.M.

    2010-11-01

    Using bulk magnetization along with elastic and inelastic neutron scattering techniques, we have investigated the phase diagram of Fe{sub 1+y}Se{sub x}Te{sub 1-x} and the nature of magnetic correlations in three nonsuperconducting samples of Fe{sub 1.01}Se{sub 0.1}Te{sub 0.9}, Fe{sub 1.01}Se{sub 0.15}Te{sub 0.85}, and Fe{sub 1.02}Se{sub 0.3}Te{sub 0.7}. A cusp and hysteresis in the temperature dependence of the magnetization for the x=0.15 and 0.3 samples indicates spin-glass (SG) ordering below T{sub sg} = 23 K. Neutron scattering measurements indicate that the spin-glass behavior is associated with short-range spin density wave (SDW) ordering characterized by a static component and a low-energy dynamic component with a characteristic incommensurate wave vector of Q{sub m} = (0.46, 0, 0.50) and an anisotropy gap of -2.5 meV. Our high Q-resolution data also show that the systems undergo a glassy structural distortion that coincides with the short-range SDW order.

  12. Skew Scattering from Correlated Systems: Impurities and Collective Excitations in the Spin Hall Effect

    Science.gov (United States)

    Ziman, Timothy; Gu, Bo; Maekawa, Sadamichi

    2017-01-01

    The spin Hall effect is affected by the Coulomb interaction as well as spin-spin correlations in metals. Here we examine the enhancement in the effect caused by resonant skew scattering induced by electron correlations. For single-impurity scattering, local Coulomb correlations may significantly change the observed spin Hall angle. There may be additional effects because of the special atomic environment close to a surface — extra degeneracies compared to the bulk, enhanced correlations that move the relative d- or f-levels, and interference effects coming from the lower local dimension. Our results may explain the very large spin Hall angle observed in CuBi alloys. We discuss the impact on the spin Hall effect from cooperative effects, firstly in an itinerant ferromagnet where there is an anomaly near the Curie temperature originating from high-order spin fluctuations. The second case considered is a metallic spin glass, where exchange via slowly fluctuating magnetic moments may lead to the precession of an injected spin current. This decreases the net spin-charge conversion from skew scattering at temperatures below a value three or four times the freezing temperature.

  13. Correlation Analysis between Spin, Velocity Shear, and Vorticity of Baryonic and Dark Matter Halos

    Science.gov (United States)

    Liu, L. L.

    2016-05-01

    Using cosmological hydrodynamic simulations, we investigate the alignments between velocity shear, vorticity, and the spin of dark matter halos, and study the correlation between baryonic and dark matter. We find that (1) mis-alignment between vorticity of baryonic and dark matter would develop on scales dark matter; (3) small/massive halos spinning parallel/perpendicular to the host filaments are sensitive to the identification of cosmic web, simulation box size, and resolution. These factors might complicate the connection between the spins of dark matter halos and galaxies, and affect the correlation signal of the alignments of galaxy spin with nearby large-scale structures.

  14. Zero-Field Magnetism of a Two-Dimensional Antiferromagnet, κ-(BEDT-TTF)2Cu[N(CN)2]Cl, Determined by Muon Spin Rotation and Magnetization Measurements

    Science.gov (United States)

    Ito, Miho; Uehara, Tomotaka; Taniguchi, Hiromi; Satoh, Kazuhiko; Ishii, Yasuyuki; Watanabe, Isao

    2015-05-01

    The zero-field magnetism of a two-dimensional noncollinear antiferromagnet, κ-(BEDT-TTF)2Cu[N(CN)2]Cl, has been investigated by magnetization and zero-field muon spin rotation (μSR) measurements. Low-field magnetization measurements enabled us to determine the magnetic transition temperature TN as 22.80 ± 0.02 K. Distinct muon spin precession signals appeared below 21.4 K. μSR spectra below 21.4 K were well described by two types of precession components and a relaxation one. The temperature dependence of internal field converted by μSR data was in good agreement with that of macroscopic residual magnetism. These results suggest that the tiny interlayer interaction, which has been suggested to be almost 106 times less than the intralayer exchange interaction, spontaneously causes the three-dimensional long-range order.

  15. Measurement of spin correlation in tt production using a matrix element approach.

    Science.gov (United States)

    Abazov, V M; Abbott, B; Acharya, B S; Adams, M; Adams, T; Alexeev, G D; Alkhazov, G; Alton, A; Alverson, G; Alves, G A; Ancu, L S; Aoki, M; Arov, M; Askew, A; Åsman, B; Atramentov, O; Avila, C; BackusMayes, J; Badaud, F; Bagby, L; Baldin, B; Bandurin, D V; Banerjee, S; Barberis, E; Baringer, P; Barreto, J; Bartlett, J F; Bassler, U; Bazterra, V; Beale, S; Bean, A; Begalli, M; Begel, M; Belanger-Champagne, C; Bellantoni, L; Beri, S B; Bernardi, G; Bernhard, R; Bertram, I; Besançon, M; Beuselinck, R; Bezzubov, V A; Bhat, P C; Bhatnagar, V; Blazey, G; Blessing, S; Bloom, K; Boehnlein, A; Boline, D; Boos, E E; Borissov, G; Bose, T; Brandt, A; Brandt, O; Brock, R; Brooijmans, G; Bross, A; Brown, D; Brown, J; Bu, X B; Buehler, M; Buescher, V; Bunichev, V; Burdin, S; Burnett, T H; Buszello, C P; Calpas, B; Camacho-Pérez, E; Carrasco-Lizarraga, M A; Casey, B C K; Castilla-Valdez, H; Chakrabarti, S; Chakraborty, D; Chan, K M; Chandra, A; Chen, G; Chevalier-Théry, S; Cho, D K; Cho, S W; Choi, S; Choudhary, B; Cihangir, S; Claes, D; Clutter, J; Cooke, M; Cooper, W E; Corcoran, M; Couderc, F; Cousinou, M-C; Croc, A; Cutts, D; Das, A; Davies, G; De, K; de Jong, S J; De la Cruz-Burelo, E; Déliot, F; Demarteau, M; Demina, R; Denisov, D; Denisov, S P; Desai, S; Deterre, C; DeVaughan, K; Diehl, H T; Diesburg, M; Dominguez, A; Dorland, T; Dubey, A; Dudko, L V; Duggan, D; Duperrin, A; Dutt, S; Dyshkant, A; Eads, M; Edmunds, D; Ellison, J; Elvira, V D; Enari, Y; Evans, H; Evdokimov, A; Evdokimov, V N; Facini, G; Ferbel, T; Fiedler, F; Filthaut, F; Fisher, W; Fisk, H E; Fortner, M; Fox, H; Fuess, S; Garcia-Bellido, A; Gavrilov, V; Gay, P; Geng, W; Gerbaudo, D; Gerber, C E; Gershtein, Y; Ginther, G; Golovanov, G; Goussiou, A; Grannis, P D; Greder, S; Greenlee, H; Greenwood, Z D; Gregores, E M; Grenier, G; Gris, Ph; Grivaz, J-F; Grohsjean, A; Grünendahl, S; Grünewald, M W; Guillemin, T; Guo, F; Gutierrez, G; Gutierrez, P; Haas, A; Hagopian, S; Haley, J; Han, L; Harder, K; Harel, A; Hauptman, J M; Hays, J; Head, T; Hebbeker, T; Hedin, D; Hegab, H; Heinson, A P; Heintz, U; Hensel, C; Heredia-De la Cruz, I; Herner, K; Hesketh, G; Hildreth, M D; Hirosky, R; Hoang, T; Hobbs, J D; Hoeneisen, B; Hohlfeld, M; Hubacek, Z; Huske, N; Hynek, V; Iashvili, I; Illingworth, R; Ito, A S; Jabeen, S; Jaffré, M; Jamin, D; Jayasinghe, A; Jesik, R; Johns, K; Johnson, M; Johnston, D; Jonckheere, A; Jonsson, P; Joshi, J; Jung, A W; Juste, A; Kaadze, K; Kajfasz, E; Karmanov, D; Kasper, P A; Katsanos, I; Kehoe, R; Kermiche, S; Khalatyan, N; Khanov, A; Kharchilava, A; Kharzheev, Y N; Khatidze, D; Kirby, M H; Kohli, J M; Kozelov, A V; Kraus, J; Kulikov, S; Kumar, A; Kupco, A; Kurča, T; Kuzmin, V A; Kvita, J; Lammers, S; Landsberg, G; Lebrun, P; Lee, H S; Lee, S W; Lee, W M; Lellouch, J; Li, L; Li, Q Z; Lietti, S M; Lim, J K; Lincoln, D; Linnemann, J; Lipaev, V V; Lipton, R; Liu, Y; Liu, Z; Lobodenko, A; Lokajicek, M; Lopes de Sa, R; Lubatti, H J; Luna-Garcia, R; Lyon, A L; Maciel, A K A; Mackin, D; Madar, R; Magaña-Villalba, R; Malik, S; Malyshev, V L; Maravin, Y; Martínez-Ortega, J; McCarthy, R; McGivern, C L; Meijer, M M; Melnitchouk, A; Menezes, D; Mercadante, P G; Merkin, M; Meyer, A; Meyer, J; Miconi, F; Mondal, N K; Muanza, G S; Mulhearn, M; Nagy, E; Naimuddin, M; Narain, M; Nayyar, R; Neal, H A; Negret, J P; Neustroev, P; Novaes, S F; Nunnemann, T; Obrant, G; Orduna, J; Osman, N; Osta, J; Otero y Garzón, G J; Padilla, M; Pal, A; Parashar, N; Parihar, V; Park, S K; Parsons, J; Partridge, R; Parua, N; Patwa, A; Penning, B; Perfilov, M; Peters, K; Peters, Y; Petridis, K; Petrillo, G; Pétroff, P; Piegaia, R; Piper, J; Pleier, M-A; Podesta-Lerma, P L M; Podstavkov, V M; Polozov, P; Popov, A V; Prewitt, M; Price, D; Prokopenko, N; Protopopescu, S; Qian, J; Quadt, A; Quinn, B; Rangel, M S; Ranjan, K; Ratoff, P N; Razumov, I; Renkel, P; Rijssenbeek, M; Ripp-Baudot, I; Rizatdinova, F; Rominsky, M; Ross, A; Royon, C; Rubinov, P; Ruchti, R; Safronov, G; Sajot, G; Salcido, P; Sánchez-Hernández, A; Sanders, M P; Sanghi, B; Santos, A S; Savage, G; Sawyer, L; Scanlon, T; Schamberger, R D; Scheglov, Y; Schellman, H; Schliephake, T; Schlobohm, S; Schwanenberger, C; Schwienhorst, R; Sekaric, J; Severini, H; Shabalina, E; Shary, V; Shchukin, A A; Shivpuri, R K; Simak, V; Sirotenko, V; Skubic, P; Slattery, P; Smirnov, D; Smith, K J; Snow, G R; Snow, J; Snyder, S; Söldner-Rembold, S; Sonnenschein, L; Soustruznik, K; Stark, J; Stolin, V; Stoyanova, D A; Strauss, M; Strom, D; Stutte, L; Suter, L; Svoisky, P; Takahashi, M; Tanasijczuk, A; Taylor, W; Titov, M; Tokmenin, V V; Tsai, Y-T; Tsybychev, D; Tuchming, B; Tully, C; Uvarov, L; Uvarov, S; Uzunyan, S; Van Kooten, R; van Leeuwen, W M; Varelas, N; Varnes, E W; Vasilyev, I A; Verdier, P; Vertogradov, L S; Verzocchi, M; Vesterinen, M; Vilanova, D; Vokac, P; Wahl, H D; Wang, M H L S; Warchol, J; Watts, G; Wayne, M; Weber, M; Welty-Rieger, L; White, A; Wicke, D; Williams, M R J; Wilson, G W; Wobisch, M; Wood, D R; Wyatt, T R; Xie, Y; Xu, C; Yacoob, S; Yamada, R; Yang, W-C; Yasuda, T; Yatsunenko, Y A; Ye, Z; Yin, H; Yip, K; Youn, S W; Yu, J; Zelitch, S; Zhao, T; Zhou, B; Zhu, J; Zielinski, M; Zieminska, D; Zivkovic, L

    2011-07-15

    We determine the fraction of tt events with spin correlation, assuming that the spin of the top quark is either correlated with the spin of the top antiquark as predicted by the standard model or is uncorrelated. For the first time we use a matrix-element-based approach to study tt spin correlation. We use tt → W+ b W- b → ℓ+ νbℓ- ν b final states produced in pp collisions at a center-of-mass energy sqrt(s)=1.96  TeV, where ℓ denotes an electron or a muon. The data correspond to an integrated luminosity of 5.4  fb(-1) and were collected with the D0 detector at the Fermilab Tevatron collider. The result agrees with the standard model prediction. We exclude the hypothesis that the spins of the tt are uncorrelated at the 97.7% C.L.

  16. Optimized resonating valence bond state in square lattice: correlations & excitations

    Directory of Open Access Journals (Sweden)

    Z Nourbakhsh

    2009-09-01

    Full Text Available We consider RVB state as a variational estimate for the ground state of Heisenberg antiferromagnet in square lattice. We present numerical calculation of energy, spin-spin correlation function and spin excitation spectrum. We show, that the quantum flactuations reduce of magnetization respect to Neel order. Our results are in good agreement with other methods such as spin-wave calculation and series expansions.

  17. Nuclear Spin Alignment and Alignment Correlation Terms in Mass A = 8 System

    Energy Technology Data Exchange (ETDEWEB)

    Sumikama, T., E-mail: sumikama@riken.jp [RIKEN (Japan); Iwakoshi, T.; Nagatomo, T.; Ogura, M.; Nakashima, Y.; Fujiwara, H.; Matsuta, K.; Minamisono, T.; Mihara, M.; Fukuda, M. [Osaka University, Department of Physics (Japan); Minamisono, K. [TRIUMF (Canada); Yamaguchi, T. [Saitama University, Department of Physics (Japan)

    2004-12-15

    The pure nuclear spin alignments of {sup 8}Li and {sup 8}B were produced from the nuclear spin polarization applying the {beta}-NMR method. The alignment correlation terms in the {beta}-ray angular distribution were observed to test the G parity conservation in the nuclear {beta} decay.

  18. Correlation of spin and structure in doped bismuth ferrite nanoparticles

    Science.gov (United States)

    Lin, J. W.; Tite, Teddy; Tang, Y. H.; Lue, C. S.; Chang, Y. M.; Lin, J. G.

    2012-04-01

    The mutiferroic Bi1-xEuxFeO3 nanoparticles with x = 0 to 0.4 are studied by x-ray diffraction (XRD), Raman spectra and electron spin resonance (ESR) with X-band (9.53 GHz), in order to investigate the doping effect on crystalline and spin structures. Both XRD and Raman spectrum reveal a structural transformation at x = 0.15, which is associated with the shortening of Bi—O bond length. These structural data are further related to the variation of ESR peak position and peak area, providing evidence for the enhancement of ferromagnetic coupling as x < 0.3.

  19. Short-range spin- and pair-correlations : a variational wave-function

    NARCIS (Netherlands)

    van der Marel, D

    2004-01-01

    A many-body wave-function is postulated, which is sufficiently general to describe superconducting pair-correlations, and/or spin-correlations, which can occur either as long-range order or as finite-range correlations. The proposed wave-function appears to summarize some of the more relevant aspect

  20. Spin Flips - II. Evolution of dark matter halo spin orientation, and its correlation with major mergers

    CERN Document Server

    Bett, Philip E

    2015-01-01

    We expand our previous study on the relationship between changes in the orientation of the angular momentum vector of dark matter haloes ("spin flips") and changes in their mass (Bett & Frenk 2012), to cover the full range of halo masses in a simulation cube of length 100 $h^{-1}$ Mpc. Since strong disturbances to a halo (such as might be indicated by a large change in the spin direction) are likely also to disturb the galaxy evolving within, spin flips could be a mechanism for galaxy morphological transformation without involving major mergers. We find that 35% of haloes have, at some point in their lifetimes, had a spin flip of at least $45\\deg$ that does not coincide with a major merger. Over 75% of large spin flips coincide with non-major mergers; only a quarter coincide with major mergers. We find a similar picture for changes to the inner-halo spin orientation, although here there is an increased likelihood of a flip occurring. Changes in halo angular momentum orientation, and other such measures of...

  1. Correlation function of four spins in the percolation model

    Directory of Open Access Journals (Sweden)

    Vladimir S. Dotsenko

    2016-10-01

    It is known that the four-point functions define the actual fusion rules of a particular model. In this respect, we find that fusion of two spins, of dimension Δσ=596, produce a new channel, in the 4-point function, which is due to the operator with dimension Δ=5/8.

  2. Measurement of ttbar Spin Correlation in ppbar Collisions Using the CDF II Detector at the Tevatron

    CERN Document Server

    al., T Aaltonen et

    2010-01-01

    The ttbar spin correlation at production is a fundamental prediction of QCD and a potentially incisive test of new physics coupled to top quarks. We measure the ttbar spin state in ppbar collisions at sqrt(s) = 1.96 TeV using 1001 candidate events in the lepton plus jets decay channel reconstructed in the CDF II detector. In the helicity basis, for a top-quark mass of 172.5 GeV/c^2, we find a spin correlation coefficient kappa = 0.60 +/- 0.50 (stat) +/- 0.16 (syst), consistent with the QCD prediction, kappa ~= 0.40.

  3. Quantum Effects in Higher-Order Correlators of a Quantum-Dot Spin Qubit

    Science.gov (United States)

    Bechtold, A.; Li, F.; Müller, K.; Simmet, T.; Ardelt, P.-L.; Finley, J. J.; Sinitsyn, N. A.

    2016-07-01

    We measure time correlators of a spin qubit in an optically active quantum dot beyond the second order. Such higher-order correlators are shown to be directly sensitive to pure quantum effects that cannot be explained within the classical framework. They allow direct determination of ensemble and quantum dephasing times, T2* and T2, using only repeated projective measurements and without the need for coherent spin control. Our method enables studies of purely quantum behavior in solid state systems, including tests of the Leggett-Garg type of inequalities that rule out local hidden variable interpretation of the quantum-dot spin dynamics.

  4. Vortical fluid and $\\Lambda$ spin correlations in high-energy heavy-ion collisions

    CERN Document Server

    Pang, Long-Gang; Wang, Qun; Wang, Xin-Nian

    2016-01-01

    Fermions become polarized in a vortical fluid due to spin-vorticity coupling. The spin polarization density is proportional to the local fluid vorticity at the next-to-leading order of a gradient expansion in a quantum kinetic theory. Spin correlations of two $\\Lambda$-hyperons can therefore reveal the vortical structure of the dense matter in high-energy heavy-ion collisions. We employ a (3+1)D viscous hydrodynamic model with event-by-event fluctuating initial conditions from A MultiPhase Transport (AMPT) model to calculate the vorticity distributions and $\\Lambda$ spin correlations. The azimuthal correlation of the transverse spin is shown to have a cosine form plus an offset due to a circular structure of the transverse vorticity around the beam direction and global spin polarization. The longitudinal spin correlation shows a structure of vortex-pairing in the transverse plane due to the convective flow of hot spots in the radial direction. The dependence on colliding energy, rapidity, centrality and sensi...

  5. The effect of four-spin exchanges on the honeycomb lattice diagram phase of S=3/2 J1-J2 Antiferromagnetic Heisenberg model

    Directory of Open Access Journals (Sweden)

    F Keshavarz

    2017-02-01

    Full Text Available In this study, the effect of four-spin exchanges between the nearest and next nearest neighbor spins of honeycomb lattice on the phase diagram of S=3/2 antiferomagnetic Heisenberg model is considered with two-spin exchanges between the nearest and next nearest neighbor spins. Firstly, the method is investigated with classical phase diagram. In classical phase diagram, in addition to Neel order, classical degeneracy is also seen. The existance of this phase in diagram phase is important because of the probability of the existence of quantum spin liquid in this region for such amount of interaction. To investigate the effect of quantum fluctuation on the stability of the obtained classical phase diagram, linear spin wave theory has been used. Obtained results show that in classical degeneracy regime, the quantum fluctuations cause the order by disorder in the spin system and the ground state is ordered

  6. Quasiparticle bandstructure of antiferromagnetic EuTe

    Science.gov (United States)

    Mathi Jaya, S.; Nolting, W.

    1997-11-01

    The temperature-dependent electronic quasiparticle spectrum of the antiferromagnetic semiconductor EuTe is derived by use of a combination of a many-body model procedure with a tight-binding - `linear muffin tin orbital' (TB - LMTO) band structure calculation. The central part is the d - f model for a single band electron (`test electron') being exchange coupled to the antiferromagnetically ordered localized moments of the Eu ions. The single-electron Bloch energies of the d - f model are taken from a TB - LMTO calculation for paramagnetic EuTe. The d - f model is evaluated by a recently proposed moment conserving Green function technique to get the temperature-dependent sublattice - quasiparticle bandstructure (S - QBS) and sublattice - quasiparticle density of states (S - QDOS) of the unoccupied 5d - 6s energy bands. Unconventional correlation effects and the appearance of characteristic quasiparticles (`magnetic polarons') are worked out in detail. The temperature dependence of the S - QDOS and S - QBS is mainly provoked by the spectral weights of the energy dispersions. Minority- and majority-spin spectra coincide for all temperatures but with different densities of states. Upon cooling from 0953-8984/9/47/012/img1 to T = 0 K the lower conduction band edge exhibits a small blue shift of -0.025 eV in accordance with the experiment. Quasiparticle damping manifesting itself in a temperature-dependent broadening of the spectral density peaks arises from spin exchange processes between (5d - 6s) conduction band electrons and localized 4f moments.

  7. Evidence for Intertwining of Superconductivity and Antiferromagnetism in a Cuprate

    Science.gov (United States)

    Tranquada, John; Xu, Zhijun; Stock, C.; Chi, S. X.; Kolesnikov, A. I.; Xu, G. Y.; Gu, G. D.

    2014-03-01

    We have used inelastic neutron scattering to measure the low-energy, incommensurate antiferromagnetic spin excitations both above and below the superconducting transition temperature (Tc = 32 K) of La1.905Ba0.095CuO4. While the magnetic excitations in optimally-doped cuprates typically show the development of a spin gap and magnetic resonance below Tc, our sample shows no such effect. Instead strong, gapless spin excitations coexist with bulk superconductivity. To understand this, we note that previous transport measurements have shown that the superconducting layers are decoupled by a magnetic field applied along the c-axis, resulting in a state with frustrated interlayer Josephson coupling, similar to LBCO with x = 1 / 8 , where it has been proposed that pair-density-wave superconductivity occurs. This suggests that, in a similar fashion, the spatially modulated antiferromagnetic correlations (which we see directly in the x = 0 . 095 sample) are intertwined with a spatially modulated superconducting pair wave function. Work at BNL supported by Office of Basic Energy Sciences, US DOE, under Contract No. DE-AC02-98CH10886.

  8. Measurement of np elastic scattering spin-spin correlation parameters at 484, 634, and 788 MeV

    Energy Technology Data Exchange (ETDEWEB)

    Garnett, R.W.

    1989-03-01

    The spin-spin correlation parameters C/sub LL/ and C/sub SL/ were measured for np elastic scattering at the incident neutron kinetic energy of 634 MeV. Good agreement was obtained with previously measured data. Additionally, the first measurement of the correlation parameter C/sub SS/ was made at the three energies, 484, 634, and 788 MeV. It was found that the new values, in general, do not agree well with phase shift predictions. A study was carried out to determine which of the isospin-0 partial waves will be affected by this new data. It was found that the /sup 1/P/sub 1/ partial wave will be affected significantly at all three measurement energies. At 634 and 788 MeV, the /sup 3/S/sub 1/ phase shifts will also change. 29 refs., 21 figs., 16 tabs.

  9. Femtosecond optomagnetism in dielectric antiferromagnets

    Science.gov (United States)

    Bossini, D.; Rasing, Th

    2017-02-01

    Optical femtosecond manipulation of magnetic order is attractive for the development of new concepts for ultrafast magnetic recording. Theoretical and experimental investigations in this research area aim at establishing a physical understanding of magnetic media in light-induced non-equilibrium states. Such a quest requires one to adjust the theory of magnetism, since the thermodynamical concepts of elementary excitations and spin alignment determined by the exchange interaction are not applicable on the femtosecond time-scale after the photo-excitation. Here we report some key milestones concerning the femtosecond optical control of spins in dielectric antiferromagnets, whose spin dynamics is by nature faster than that of ferromagnets and can be triggered even without any laser heating. The recent progress of the opto-magnetic effect in the sub-wavelength regime makes this exciting research area even more promising, in terms of both fundamental breakthroughs and technological perspectives.

  10. Spatially anisotropic Heisenberg kagome antiferromagnet

    Science.gov (United States)

    Apel, W.; Yavors'kii, T.; Everts, H.-U.

    2007-04-01

    In the search for spin-1/2 kagome antiferromagnets, the mineral volborthite has recently been the subject of experimental studies (Hiroi et al 2001 J. Phys. Soc. Japan 70 3377; Fukaya et al 2003 Phys. Rev. Lett. 91 207603; Bert et al 2004 J. Phys.: Condens. Matter 16 S829; Bert et al 2005 Phys. Rev. Lett. 95 087203). It has been suggested that the magnetic properties of this material are described by a spin-1/2 Heisenberg model on the kagome lattice with spatially anisotropic exchange couplings. We report on investigations of the {\\mathrm {Sp}}(\\mathcal {N}) symmetric generalization of this model in the large \\mathcal {N} limit. We obtain a detailed description of the dependence of possible ground states on the anisotropy and on the spin length S. A fairly rich phase diagram with a ferrimagnetic phase, incommensurate phases with and without long-range order and a decoupled chain phase emerges.

  11. Studies of spin-orbit correlations at JLAB

    Energy Technology Data Exchange (ETDEWEB)

    Mher Aghasyan, Harut Avakian

    2011-05-01

    Studies of single spin asymmetries for pion electroproduction in semi-inclusive deep-inelastic scattering are presented using the polarized \\sim6 GeV electrons from at the Thomas Jefferson National Accelerator Facility (JLab) and the Continuous Electron Beam Accelerator Facility (CEBAF) Large Acceptance Spectrometer (CLAS) with the Inner Calorimeter. The cross section versus the azimuthal angle {\\phi}_h of the produced neutral pion has a substantial sin {\\phi}_h amplitude. The dependence of this amplitude on Bjorken x_B and on the pion transverse momentum is extracted and compared with published data.

  12. Measurement of Spin Correlation in Top Quark Pair Production in Semi-Leptonic Final State

    CERN Document Server

    Baarmand, Marc M; Vodopiyanov, Igor

    2006-01-01

    The measurement of correlation between spins of top and anti-top quarks, produced in proton-proton collisions at LHC, is described for the semi-leptonic decay of the top quark pair (one top quark decaying leptonically and the other hadronically). The simulated events are reconstructed after full simulation of the CMS detector. The spin correlation coefficient is estimated based on a total integrated luminosity of ten inverse femtobarns. Including systematic uncertainties, the correlation coefficient can be measured with a total relative uncertainty of 17% or 27% depending on the choice of the deay angles used.

  13. Photon Spin and the Shape of the Two-Photon Correlation Function

    CERN Document Server

    Slotta, C; Slotta, Claus; Heinz, Ulrich

    1997-01-01

    We use the covariant current formalism to derive the general form of the 2-photon correlation function for fully chaotic sources. Motivated by the recent discussion in the literature we concentrate on the effects from the photon spin on the correlator. We show that for locally thermalized expanding sources, like those expected to be created in relativistic heavy ion collisions, the only change relative to 2-pion interferometry is a statistical factor 1/2 for the overall strength of the correlation which results from the experimental averaging over the photon spin.

  14. Lattice distortion in disordered antiferromagnetic XY models

    Institute of Scientific and Technical Information of China (English)

    Li Peng-Fei; Cao Hai-Jing

    2012-01-01

    The behavior of lattice distortion in spin 1/2 antiferromagnetic XY models with random magnetic modulation is investigated with the consideration of spin-phonon coupling in the adiabatic limit.It is found that lattice distortion relies on the strength of the random modulation.For strong or weak enough spin-phonon couplings,the average lattice distortion may decrease or increase as the random modulation is strengthened.This may be the result of competition between the random magnetic modulation and the spin-phonon coupling.

  15. Inclusive Single-Spin Asymmetries, Quark-Photon, and Quark-Quark Correlations

    CERN Document Server

    Burkardt, Matthias

    2016-01-01

    We consider quark-photon correlations that have been proposed as a source for single-spin asymmetries in inclusive deep-inelastic scattering. A new sum rule for these correlators is derived and its phenomenological consequences are discussed. The results are interpreted within the context of an intuitive 'electrodynamic lensing' picture.

  16. Internal energy and specific heat in a ferromagnetic-antiferromagnetic double layers

    Institute of Scientific and Technical Information of China (English)

    Jiang Wei; Guo An-Bang

    2007-01-01

    The internal energy and specific heat of a Heisenberg ferro- antiferromagnetic double-layer system are studied by using spin-wave theory and the retarded Green function method at low temperatures. Numerical results show that the antiferromagnetic intralayer coupling J2 has an important influence on internal energy and specific heat for a four-sublattice system with antiferromagnetic (or ferrimagnetic) interlayer couplings.

  17. Correlation functions of the spin chains. Algebraic Bethe Ansatz approach; Fonctions de correlation des chaines de spin. Approche de l'ansatz de Bethe algebrique

    Energy Technology Data Exchange (ETDEWEB)

    Kitanine, N

    2007-09-15

    Spin chains are the basic elements of integrable quantum models. These models have direct applications in condense matter theory, in statistical physics, in quantum optics, in field theory and even in string theory but they are also important because they enable us to solve, in an exact manner, non-perturbative phenomena that otherwise would stay unresolved. The method described in this work is based on the algebraic Bethe Ansatz. It is shown how this method can be used for the computation of null temperature correlation functions of the Heisenberg 1/2 spin chain. The important point of this approach is the solution of the inverse quantum problem given by the XXZ spin chain. This solution as well as a simple formulae for the scalar product of the Bethe states, have enabled us to get the most basic correlation functions under the form of multiple integrals. The formalism of multiple integrals open the way for asymptotic analysis for a few physical quantities like the probability of vacuum formation. It is worth noticing that this formalism can give exact results for two-point functions that are the most important correlation functions for applications. A relationship has been discovered between these multiple integrals and the sum of the form factors. The results have been extended to dynamical correlation functions. (A.C.)

  18. Thermodynamic properties of correlated fermions in lattices with spin-dependent disorder

    Science.gov (United States)

    Makuch, K.; Skolimowski, J.; Chakraborty, P. B.; Byczuk, K.; Vollhardt, D.

    2013-04-01

    Motivated by the rapidly growing possibilities for experiments with ultracold atoms in optical lattices, we investigate the thermodynamic properties of correlated lattice fermions in the presence of an external spin-dependent random potential. The corresponding model, a Hubbard model with spin-dependent local random potentials, is solved within dynamical mean-field theory. This allows us to present a comprehensive picture of the thermodynamic properties of this system. In particular, we show that for a fixed total number of fermions spin-dependent disorder induces a magnetic polarization. The magnetic response of the polarized system differs from that of a system with conventional disorder.

  19. Interplay between spin-orbit coupling and strong correlation effects: Comparison of the three osmate double perovskites Ba2A OsO6 (A =Na , Ca, Y)

    Science.gov (United States)

    Gangopadhyay, Shruba; Pickett, Warren E.

    2016-04-01

    High formal valence Os-based double perovskites are a focus of current interest because they display strong interplay of large spin-orbit coupling and strong electronic correlation. Here we present the electronic and magnetic characteristics of a sequence of three cubic Os based double perovskites Ba2A OsO6 (A =Na , Ca, Y), with formal valences of Os +7(d1) ,Os +6(d2) , and Os +5(d3) . For these first principles based calculations we apply an "exact exchange for correlated electrons" functional, with exact exchange applied in a hybrid fashion solely to the Os (5 d ) states. While Ba2NaOsO6 is a reported ferromagnetic Dirac-Mott insulator studied previously, the other two show antiferromagnetic ordering while all retain the undistorted cubic structure. For comparison purposes we have investigated only the ferromagnetic ordered phase. A metal-insulator transition is predicted to occur upon rotating the direction of magnetization in all three materials, reflecting the central role of spin-orbit coupling in these small gap osmates. Surprises arising from comparing formal charge states with the radial charge densities are discussed. Chemical shielding factors and orbital susceptibilities are provided for comparison with future nuclear magnetic resonance data.

  20. New insights into electron spin dynamics in the presence of correlated noise.

    Science.gov (United States)

    Spezia, S; Adorno, D Persano; Pizzolato, N; Spagnolo, B

    2012-02-08

    The changes in the spin depolarization length in zinc-blende semiconductors when an external component of correlated noise is added to a static driving electric field are analyzed for different values of field strength, noise amplitude and correlation time. Electron dynamics is simulated by a Monte Carlo procedure which takes into account all the possible scattering phenomena of the hot electrons in the medium and includes the evolution of spin polarization. Spin depolarization is studied by examining the decay of the initial spin polarization of the conduction electrons through the D'yakonov-Perel process, the only relevant relaxation mechanism in III-V crystals. Our results show that, for electric field amplitudes lower than the Gunn field, the dephasing length shortens with increasing noise intensity. Moreover, a nonmonotonic behavior of spin depolarization length with the noise correlation time is found, characterized by a maximum variation for values of noise correlation time comparable with the dephasing time. Instead, in high field conditions, we find that, critically depending on the noise correlation time, external fluctuations can positively affect the relaxation length. The influence of the inclusion of the electron-electron scattering mechanism is also shown and discussed.

  1. The electronic structure of antiferromagnetic chromium

    DEFF Research Database (Denmark)

    Skriver, Hans Lomholt

    1981-01-01

    The author has used the local spin density formalism to perform self-consistent calculations of the electronic structure of chromium in the non-magnetic and commensurate antiferromagnetic phases, as a function of the lattice parameter. A change of a few per cent in the atomic radius brings...

  2. Antiferromagnetic Ising model on the swedenborgite lattice

    NARCIS (Netherlands)

    Buhrandt, Stefan; Fritz, Lars

    2014-01-01

    Geometrical frustration in spin systems often results in a large number of degenerate ground states. In this work, we study the antiferromagnetic Ising model on the three-dimensional swedenborgite lattice, which is a specific stacking of kagome and triangular layers. The model contains two exchange

  3. Transverse spin and momentum correlations in quantum chromodynamics

    Indian Academy of Sciences (India)

    Leonard P Gamberg

    2009-01-01

    The naive time reversal odd (`T-odd') parton distribution and fragmentation functions are explored. We use the spectator model framework to study flavour dependence of the Boer–Mulders $(h_{1}^{⊥})$ and Sivers $(f_{1\\text{T}}^{⊥})$ functions as well as the `T-even' but chiral odd function $h_{1\\text{L}}^{⊥}$. These transverse momentum-dependent parton distribution functions are of significance for the analysis of azimuthal asymmetries in semi-inclusive deep inelastic scattering, as well as for the overall physical understanding of the distribution of transversely polarized quarks in unpolarized hadrons. In this context we also consider the Collins mechanism and the fragmentation function $H_{1}^{⊥}$. As a by-product of this analysis we calculate the leading twist unpolarized cos(2) asymmetry, and sin(2) single spin asymmetry for a longitudinally polarized target in semi-inclusive deep inelastic scattering.

  4. Quasiparticle excitations in frustrated antiferromagnets

    Energy Technology Data Exchange (ETDEWEB)

    Trumper, Adolfo E. [Instituto de Fisica Rosario (CONICET) Universidad Nacional de Rosario, Boulevard 27 de Febrero 210 bis, 2000 Rosario (Argentina)]. E-mail: trumper@ifir.edu.ar; Gazza, Claudio J. [Instituto de Fisica Rosario (CONICET) Universidad Nacional de Rosario, Boulevard 27 de Febrero 210 bis, 2000 Rosario (Argentina); Manuel, Luis O. [Instituto de Fisica Rosario (CONICET) Universidad Nacional de Rosario, Boulevard 27 de Febrero 210 bis, 2000 Rosario (Argentina)]. E-mail: manuel@ifir.edu.ar

    2004-12-31

    We have computed the quasiparticle wave function corresponding to a hole injected in a triangular antiferromagnet. We have taken into account multi-magnon contributions within the self-consistent Born approximation. We have found qualitative differences, under sign reversal of the integral transfer t, regarding the multi-magnon components and the own existence of the quasiparticle excitations. Such differences are due to the subtle interplay between magnon-assisted and free hopping mechanisms. We conclude that the conventional quasiparticle picture can be broken by geometrical frustration without invoking spin liquid phases.

  5. Communication: Configuration interaction combined with spin-projection for strongly correlated molecular electronic structures

    Energy Technology Data Exchange (ETDEWEB)

    Tsuchimochi, Takashi, E-mail: tsuchimochi@gmail.com; Ten-no, Seiichiro, E-mail: tenno@garnet.kobe-u.ac.jp [Graduate School of System Informatics, Kobe University, Kobe 657-8501 (Japan)

    2016-01-07

    We present single and double particle-hole excitations in the recently revived spin-projected Hartree-Fock. Our motivation is to treat static correlation with spin-projection and recover the residual correlation, mostly dynamic in nature, with simple configuration interaction (CI). To this end, we introduce the Wick theorem for nonorthogonal determinants, which enables an efficient implementation in conjunction with the direct CI scheme. The proposed approach, termed spin-extended CI with singles and doubles, achieves a balanced treatment between dynamic and static correlations. To approximately account for the quadruple excitations, we also modify the well-known Davidson correction. We report that our approaches yield surprisingly accurate potential curves for HF, H{sub 2}O, N{sub 2}, and a hydrogen lattice, compared to traditional single reference wave function methods at the same computational scaling as regular CI.

  6. Measurement of the transverse spin correlations in the decay $Z \\rightarrow \\tau^+\\tau^-$

    CERN Document Server

    Barate, R; Décamp, D; Ghez, P; Goy, C; Lees, J P; Lucotte, A; Minard, M N; Nief, J Y; Pietrzyk, B; Casado, M P; Chmeissani, M; Comas, P; Crespo, J M; Delfino, M C; Fernández, E; Fernández-Bosman, M; Garrido, L; Juste, A; Martínez, M; Miquel, R; Mir, L M; Orteu, S; Padilla, C; Park, I C; Pascual, A; Perlas, J A; Riu, I; Sánchez, F; Teubert, F; Colaleo, A; Creanza, D; De Palma, M; Gelao, G; Iaselli, Giuseppe; Maggi, G; Maggi, M; Marinelli, N; Nuzzo, S; Ranieri, A; Raso, G; Ruggieri, F; Selvaggi, G; Silvestris, L; Tempesta, P; Tricomi, A; Zito, G; Huang, X; Lin, J; Ouyang, Q; Wang, T; Xie, Y; Xu, R; Xue, S; Zhang, J; Zhang, L; Zhao, W; Abbaneo, D; Alemany, R; Becker, U; Bazarko, A O; Bright-Thomas, P G; Cattaneo, M; Cerutti, F; Dissertori, G; Drevermann, H; Forty, Roger W; Frank, M; Hagelberg, R; Hansen, J B; Harvey, J; Janot, P; Jost, B; Kneringer, E; Knobloch, J; Lehraus, Ivan; Lutters, G; Mato, P; Minten, Adolf G; Moneta, L; Pacheco, A; Pusztaszeri, J F; Ranjard, F; Rizzo, G; Rolandi, Luigi; Rousseau, D; Schlatter, W D; Schmitt, M; Schneider, O; Tejessy, W; Tomalin, I R; Wachsmuth, H W; Wagner, A; Ajaltouni, Ziad J; Barrès, A; Boyer, C; Falvard, A; Ferdi, C; Gay, P; Guicheney, C; Henrard, P; Jousset, J; Michel, B; Monteil, S; Montret, J C; Pallin, D; Perret, P; Podlyski, F; Proriol, J; Rosnet, P; Rossignol, J M; Fearnley, Tom; Hansen, J D; Hansen, J R; Hansen, P H; Nilsson, B S; Rensch, B; Wäänänen, A; Daskalakis, G; Kyriakis, A; Markou, C; Simopoulou, Errietta; Siotis, I; Vayaki, Anna; Blondel, A; Bonneaud, G R; Brient, J C; Bourdon, P; Rougé, A; Rumpf, M; Valassi, Andrea; Verderi, M; Videau, H L; Candlin, D J; Parsons, M I; Focardi, E; Parrini, G; Zachariadou, K; Corden, M; Georgiopoulos, C H; Jaffe, D E; Antonelli, A; Bencivenni, G; Bologna, G; Bossi, F; Campana, P; Capon, G; Casper, David William; Chiarella, V; Felici, G; Laurelli, P; Mannocchi, G; Murtas, F; Murtas, G P; Passalacqua, L; Pepé-Altarelli, M; Curtis, L; Dorris, S J; Halley, A W; Knowles, I G; Lynch, J G; O'Shea, V; Raine, C; Scarr, J M; Smith, K; Teixeira-Dias, P; Thompson, A S; Thomson, E; Thomson, F; Turnbull, R M; Geweniger, C; Graefe, G; Hanke, P; Hansper, G; Hepp, V; Kluge, E E; Putzer, A; Schmidt, M; Sommer, J; Tittel, K; Werner, S; Wunsch, M; Beuselinck, R; Binnie, David M; Cameron, W; Dornan, Peter J; Girone, M; Goodsir, S M; Martin, E B; Moutoussi, A; Nash, J; Sedgbeer, J K; Spagnolo, P; Stacey, A M; Williams, M D; Ghete, V M; Girtler, P; Kuhn, D; Rudolph, G; Betteridge, A P; Bowdery, C K; Colrain, P; Crawford, G; Finch, A J; Foster, F; Hughes, G; Jones, R W L; Sloan, Terence; Williams, M I; Galla, A; Giehl, I; Greene, A M; Hoffmann, C; Jakobs, K; Kleinknecht, K; Quast, G; Renk, B; Rohne, E; Sander, H G; Van Gemmeren, P; Zeitnitz, C; Aubert, Jean-Jacques; Benchouk, C; Bonissent, A; Bujosa, G; Calvet, D; Carr, J; Coyle, P; Diaconu, C A; Etienne, F; Konstantinidis, N P; Leroy, O; Motsch, F; Payre, P; Talby, M; Sadouki, A; Thulasidas, M; Trabelsi, K; Aleppo, M; Ragusa, F; Berlich, R; Blum, Walter; Büscher, V; Dietl, H; Ganis, G; Gotzhein, C; Kroha, H; Lütjens, G; Lutz, Gerhard; Männer, W; Moser, H G; Richter, R H; Rosado-Schlosser, A; Schael, S; Settles, Ronald; Seywerd, H C J; Saint-Denis, R; Stenzel, H; Wiedenmann, W; Wolf, G; Boucrot, J; Callot, O; Chen, S; Choi, Y; Cordier, A; Davier, M; Duflot, L; Grivaz, J F; Heusse, P; Höcker, A; Jacholkowska, A; Jacquet, M; Kim, D W; Le Diberder, F R; Lefrançois, J; Lutz, A M; Nikolic, I A; Schune, M H; Simion, S; Tournefier, E; Veillet, J J; Videau, I; Zerwas, D; Azzurri, P; Bagliesi, G; Batignani, G; Bettarini, S; Bozzi, C; Calderini, G; Carpinelli, M; Ciocci, M A; Ciulli, V; Dell'Orso, R; Fantechi, R; Ferrante, I; Foà, L; Forti, F; Giassi, A; Giorgi, M A; Gregorio, A; Ligabue, F; Lusiani, A; Marrocchesi, P S; Messineo, A; Palla, Fabrizio; Sanguinetti, G; Sciabà, A; Steinberger, Jack; Tenchini, Roberto; Tonelli, G; Vannini, C; Venturi, A; Verdini, P G; Blair, G A; Bryant, L M; Chambers, J T; Gao, Y; Green, M G; Medcalf, T; Perrodo, P; Strong, J A; Von Wimmersperg-Töller, J H; Botterill, David R; Clifft, R W; Edgecock, T R; Haywood, S; Maley, P; Norton, P R; Thompson, J C; Wright, A E; Bloch-Devaux, B; Colas, P; Emery, S; Kozanecki, Witold; Lançon, E; Lemaire, M C; Locci, E; Pérez, P; Rander, J; Renardy, J F; Roussarie, A; Schuller, J P; Schwindling, J; Trabelsi, A; Vallage, B; Black, S N; Dann, J H; Johnson, R P; Kim, H Y; Litke, A M; McNeil, M A; Taylor, G; Booth, C N; Boswell, R; Brew, C A J; Cartwright, S L; Combley, F; Kelly, M S; Lehto, M H; Newton, W M; Reeve, J; Thompson, L F; Böhrer, A; Brandt, S; Cowan, G D; Grupen, Claus; Saraiva, P; Smolik, L; Stephan, F; Apollonio, M; Bosisio, L; Della Marina, R; Giannini, G; Gobbo, B; Musolino, G; Rothberg, J E; Wasserbaech, S R; Armstrong, S R; Charles, E; Elmer, P; Ferguson, D P S; González, S; Greening, T C; Hayes, O J; Hu, H; Jin, S; McNamara, P A; Nachtman, J M; Nielsen, J; Orejudos, W; Pan, Y B; Saadi, Y; Scott, I J; Walsh, J; Wu Sau Lan; Wu, X; Yamartino, J M; Zobernig, G

    1997-01-01

    For tau leptons produced in e^+e^- -> tau^+ tau^- interactions there are, in addition to the longitudinal spin correlations, two independent transverse spin correlations associated with the transverse (within the production plane) and normal (to the production plane) polarization components. A measurement of the transverse-transverse and transverse-normal tau spin correlations in the decay Z -> tau^+ tau^-, C_{TT} and C_{TN}, is presented based on the aplanarity angle of the decay products of both tau leptons. Using 80 pb^{-1} of data collected by ALEPH on the peak of the Z resonance, the results are C_{TT} = 1.06 +- 0.13 (stat) +- 0.05 (syst), and C_{TN} = 0.08 +- 0.13 (stat) +- 0.04 (syst). These values are in agreement with the Standard Model predictions, C_{TT} = 0.99 and C_{TN} = -0.01.

  7. Ba8CoNb6O24 : A spin-1/2 triangular-lattice Heisenberg antiferromagnet in the two-dimensional limit

    Science.gov (United States)

    Rawl, R.; Ge, L.; Agrawal, H.; Kamiya, Y.; Dela Cruz, C. R.; Butch, N. P.; Sun, X. F.; Lee, M.; Choi, E. S.; Oitmaa, J.; Batista, C. D.; Mourigal, M.; Zhou, H. D.; Ma, J.

    2017-02-01

    The perovskite Ba8CoNb6O24 comprises equilateral effective spin-1/2 Co2 + triangular layers separated by six nonmagnetic layers. Susceptibility, specific heat, and neutron scattering measurements combined with high-temperature series expansions and spin-wave calculations confirm that Ba8CoNb6O24 is basically a two-dimensional magnet with no detectable spin anisotropy and no long-range magnetic ordering down to 0.06 K. In other words, Ba8CoNb6O24 is very close to be a realization of the paradigmatic spin-1/2 triangular Heisenberg model, which is not expected to exhibit symmetry breaking at finite temperatures according to the Mermin and Wagner theorem.

  8. Time-domain shape of electron spin echo signal of spin-correlated radical pairs in polymer/fullerene blends

    Science.gov (United States)

    Popov, Alexander A.; Lukina, Ekaterina A.; Rapatskiy, Leonid; Kulik, Leonid V.

    2017-03-01

    Temporal shape of electron spin echo (ESE) signal of photoinduced spin-correlated radical pairs (SCRP) in composite of conductive polymer P3HT and substituted fullerene PCBM is studied in details. ESE signals of radical pairs (RP) P3HT+/PCBM- are calculated in realistic model, taking into account finite microwave pulse length. Inhomogeneous broadening of resonant lines and interradical distance distribution are included. Experimentally observed ESE time-domain shape was found to contradict predictions of conventional SCRP theory, which would be valid in the case of very fast electron transfer. Thus, instantaneous formation of singlet SCRP is not the case for P3HT+/PCBM- pair, and spin system has enough time to evolve coherently during sequential electron transfer. While it is impossible to reproduce experimental data within simple singlet SCRP model, assumption of presence of additional - with respect to what is predicted by singlet SCRP theory - AE (absorption/emission) spin polarization gives convincing accordance with the experiment. Density matrix of RP P3HT+/PCBM- is a superposition of two contributions, namely the parts reflecting (i) antiphase polarization of original singlet-born SCRP and (ii) additional AE-polarization which is generated during initial stage of charge separation. AE-polarization affects experimental ESEEM (electron spin echo envelope modulation) traces, as well as ESE shape, making impossible their interpretation via simple singlet SCRP model. However, this effect can be eliminated by averaging of ESEEM traces over EPR spectral positions. Finally, choosing the optimal gate for ESE time-domain integration and proper microwave detection phase tuning are considered.

  9. Quantum phase diagram of distorted J 1 - J 2 Heisenberg S  =  1/2 antiferromagnet in honeycomb lattice: a modified spin wave study.

    Science.gov (United States)

    Ghorbani, Elaheh; Shahbazi, Farhad; Mosadeq, Hamid

    2016-10-12

    Using the modified spin wave method, we study the [Formula: see text] Heisenberg model with first and second neighbor antiferromagnetic exchange interactions. For a symmetric S  =  1/2 model, with the same couplings for all the equivalent neighbors, we find three phases in terms of the frustration parameter [Formula: see text]: (1) a commensurate collinear ordering with staggered magnetization (Néel.I state) for [Formula: see text], (2) a magnetically gapped disordered state for [Formula: see text], preserving all the symmetries of the Hamiltonian and lattice, which by definition is a quantum spin liquid (QSL) state and (3) a commensurate collinear ordering in which two out of the three nearest neighbor magnetizations are antiparallel and the remaining pair are parallel (Néel.II state), for [Formula: see text]. We also explore the phase diagram of a distorted [Formula: see text] model with S  =  1/2. Distortion is introduced as an inequality of one nearest neighbor coupling with the other two. This yields a richer phase diagram by the appearance of a new gapped QSL, a gapless QSL and also a valence bond crystal phase in addition to the previous three phases found for the undistorted model.

  10. Quantum phase diagram of distorted J 1 - J 2 Heisenberg S  =  1/2 antiferromagnet in honeycomb lattice: a modified spin wave study

    Science.gov (United States)

    Ghorbani, Elaheh; Shahbazi, Farhad; Mosadeq, Hamid

    2016-10-01

    Using the modified spin wave method, we study the {{J}1}-{{J}2} Heisenberg model with first and second neighbor antiferromagnetic exchange interactions. For a symmetric S  =  1/2 model, with the same couplings for all the equivalent neighbors, we find three phases in terms of the frustration parameter \\barα={{J}2}/{{J}1} : (1) a commensurate collinear ordering with staggered magnetization (Néel.I state) for 0≤slant \\barα≲ 0.207 , (2) a magnetically gapped disordered state for 0.207≲ \\barα≲ 0.369 , preserving all the symmetries of the Hamiltonian and lattice, which by definition is a quantum spin liquid (QSL) state and (3) a commensurate collinear ordering in which two out of the three nearest neighbor magnetizations are antiparallel and the remaining pair are parallel (Néel.II state), for 0.396≲ \\barα≤slant 1 . We also explore the phase diagram of a distorted {{J}1}-{{J}2} model with S  =  1/2. Distortion is introduced as an inequality of one nearest neighbor coupling with the other two. This yields a richer phase diagram by the appearance of a new gapped QSL, a gapless QSL and also a valence bond crystal phase in addition to the previous three phases found for the undistorted model.

  11. Correlation Inequalities for Spin Glass in one Dimension

    CERN Document Server

    Contucci, Pierluigi

    2007-01-01

    We prove two inequalities for the direct and truncated correlation for the nearest-neighboor one-dimensional Edwards-Anderson model with symmetric quenched disorder. The second inequality has the opposite sign of the GKS inequality of type II. In the non symmetric case with positive average we show that while the direct correlation keeps its sign the truncated one changes sign when crossing a suitable line in the parameter space. That line separates the regions satisfying the GKS second inequality and the one proved here.

  12. Correlations between the dynamics of parallel tempering and the free-energy landscape in spin glasses

    Science.gov (United States)

    Yucesoy, Burcu; Machta, Jonathan; Katzgraber, Helmut G.

    2013-01-01

    We present the results of a large-scale numerical study of the equilibrium three-dimensional Edwards-Anderson Ising spin glass with Gaussian disorder. Using parallel tempering (replica exchange) Monte Carlo we measure various static, as well as dynamical quantities, such as the autocorrelation times and round-trip times for the parallel tempering Monte Carlo method. The correlation between static and dynamic observables for 5000 disorder realizations and up to 1000 spins down to temperatures at 20% of the critical temperature is examined. Our results show that autocorrelation times are directly correlated with the roughness of the free-energy landscape.

  13. Angles and Daemons: Spin Correlations at the LHC

    Energy Technology Data Exchange (ETDEWEB)

    Tran, Nhan V. [Johns Hopkins Univ., Baltimore, MD (United States)

    2011-09-01

    The Large Hadron Collider has recently started collecting data, opening a new energy regime. This will allow us to probe further than ever before many of the current mysteries of the field. New physics beyond the Standard Model, the field's current paradigm, could manifest itself via new particles. In addition, the Higgs boson, hypothesized as a consequence of electroweak symmetry breaking, remains undiscovered. At the time of discovery, the properties of such particles will be unknown. In order to understand the nature of any new physics, it will be important to understand the properties of that new particle. Methods are presented for measuring its spin, parity and coupling to the Standard Model particles. These methods are implemented at the Compact Muon Solenoid experiment and an analysis is presented with the data collected during 2010 and 2011 running at the Large Hadron Collider. An application of these techniques is used to make a measurement of the weak mixing angle. A current status of the search for the Higgs boson is also presented.

  14. The f-spin physics of rare-earth iron pnictides: influence of d-electron antiferromagnetic order on heavy fermion phase diagram

    Energy Technology Data Exchange (ETDEWEB)

    Zhu, Jian-xin [Los Alamos National Laboratory; Dai, Jianhui [ZHEJIANG UNIV; Si, Qimiao [RICE UNIV

    2009-01-01

    Some of the high {Tc} iron pnictides contain rare-earth elements, raising the question of how the existence and tunability of a d-electron antiferromagnetic order influences the heavy fermion behavior of the f-moments. With CeOFeP and CeOFeAs in mind as prototypes, we derive an extended Anderson lattice model appropriate for these quaternary systems. We show that the Kondo screening of the f-moments are efficiently suppressed by the d-electron ordering. We also argue that, inside the d-electron ordered state (as in CeOFeAs), the f-moments provide a rare realization of a quantum frustrated magnet with competing J{sub 1}-J{sub 2}-J{sub 3} interactions in an effective square lattice. Implications ofr the heavy fermion physics in broader contexts are also discussed.

  15. Energy transfer and correlation dynamics in a three-quasi-spin-pigment system

    Institute of Scientific and Technical Information of China (English)

    Zhang Yin-Ping; Li Hong-Rong; Fang Ai-Ping; Chen Hao; Li Fu-Li

    2013-01-01

    In this paper,the effects of quantum and classical correlations on the excitation energy transfer in a three-quasi-spin-pigment system are investigated.We first study the dependence of the energy transfer efficiency on various initial correlations of the donor pigments,and find that the initial concurrence is crucial to the efficiency no matter whether the initial states are pure or mixed.We then demonstrate the dynamics of correlations of the system and observe the appearance of sudden death of quantum correlations in the donor pigments.The relation between the energy transfer efficiency and the dynamics of correlations in the donor pigments is also discussed.

  16. Correlation driven charge and spin fluctuations in LaCoO{sub 3}

    Energy Technology Data Exchange (ETDEWEB)

    Karolak, Michael [Institut fuer Theoretische Physik und Astrophysik, Universitaet Wuerzburg, Am Hubland, 97074 Wuerzburg (Germany); Izquierdo, Manuel [European XFEL GmbH, Albert-Einstein-Ring 19, 22761 Hamburg (Germany); Synchrotron Soleil, L' Orme des Merisiers St-Aubin, BP-48, 91192, Gif-sur-Yvette (France); Institut fuer Theoretische Physik, Universitaet Hamburg, Jungiusstrasse 9, 20355 Hamburg (Germany); Molodtsov, Serguei L. [European XFEL GmbH, Albert-Einstein-Ring 19, 22761 Hamburg (Germany); Institute of Experimental Physics, Technische Universitaet Bergakademie Freiberg, 09599 Freiberg (Germany); ITMO University, Kronverkskiy pr. 49, 197101 St. Petersburg (Russian Federation); Lichtenstein, Alexander I. [Institut fuer Theoretische Physik, Universitaet Hamburg, Jungiusstrasse 9, 20355 Hamburg (Germany)

    2015-07-01

    The spin transition in LaCoO{sub 3} has been investigated within the DFT+DMFT formalism using continuous time quantum Monte Carlo. Calculations on the experimental rhombohedral atomic structure with two Co sites per unit cell show that an independent treatment of the Co atoms results in a ground state with charge imbalance induced by electronic correlations. Each atom shows a contribution from either a d{sup 5} or a d{sup 7} state in addition to the main d{sup 6} state. These charged states play a relevant role in the spin transition which can be understood as a low spin-high spin (LS-HS) transition with significant contributions (∝ 10%) to the LS and HS states of d{sup 5} and d{sup 7} states. A thermodynamic analysis reveals that the introduction of charge imbalance significantly lowers the total energy of the system.

  17. A novel method for measurement of the spin correlation function for relativistic electron pairs produced in Møller scattering

    Science.gov (United States)

    Bodek, K.; Kępka, D.; Rozpędzik, D.; Zejma, J.; Kozela, A.

    2017-04-01

    A self-calibrating double-Mott polarimeter is proposed for measurement of the spin correlation function of relativistic electron pairs produced in Møller scattering. The polarization of outgoing electrons (appearing when the beam is polarized) is utilized for calibration of effective analyzing powers in the secondary Mott scattering used for spin analysis. The experiment will measure the newly introduced relative spin correlation function. This new observable can be measured with a significantly better accuracy than the regular spin correlation function in a small scale experiment. It is shown that both the spin correlation function and the relative spin correlation function are theoretically equivalent. A specific experimental data analysis scenario is proposed, which effectively eliminates the systematic effects related to the imperfect geometry and detector efficiency.

  18. Noise and current correlations in tunnel junctions of quantum spin Hall edge states

    Science.gov (United States)

    Dolcini, Fabrizio

    2015-10-01

    The edge channels of two-dimensional topological systems are protected from elastic reflection and are noiseless at low temperature. Yet, noise and cross correlations can be induced when electron waves partly transmit to the opposite edge via tunneling through a constriction. In particular, in a quantum spin Hall (QSH) system tunneling occurs via both spin-preserving (p ) and spin-flipping (f ) processes, each fulfilling time-reversal symmetry. We investigate the current correlations of a four-terminal QSH setup in the presence of a tunneling region, both at equilibrium and out of equilibrium. We find that, although p and f processes do not commute and the generic current correlation depends on both, under appropriate conditions a direct detection of two types of partition noise is possible. In particular, while the spin-preserving partitioning can be probed for any arbitrary tunnel junction with a specific configuration of terminal biases, the spin-flipping partitioning can be directly detected only under suitably designed setups and conditions. We describe two setups where these conditions can be fulfilled, and both types of partitioning can be detected and controlled.

  19. Time-Correlated Structure in Spin Fluctuations in Pulsars

    CERN Document Server

    Price, Steve; Shore, Steve; Nice, David

    2012-01-01

    We study statistical properties of stochastic variations in pulse arrival times, timing noise, in radio pulsars using a new analysis method applied in the time domain. The method proceeds in two steps. First, we subtract low-frequency wander using a high-pass filter. Second, we calculate the discrete correlation function of the filtered data. As a complementary method for measuring correlations, we introduce a statistic that measures the dispersion of the data with respect to the data translated in time. The analysis methods presented here are robust and of general usefulness for studying arrival time variations over timescales approaching the average sampling interval. We apply these methods to timing data for 32 pulsars. In two radio pulsars, PSRs B1133+16 and B1933+16, we find that fluctuations in arrival times are correlated over timescales of 10 - 20 d with the distinct signature of a relaxation process. Though this relaxation response could be magnetospheric in origin, we argue that damping between the ...

  20. An hour-glass magnetic spectrum in an insulating, hole-doped antiferromagnet.

    Science.gov (United States)

    Boothroyd, A T; Babkevich, P; Prabhakaran, D; Freeman, P G

    2011-03-17

    Superconductivity in layered copper oxide compounds emerges when charge carriers are added to antiferromagnetically ordered CuO(2) layers. The carriers destroy the antiferromagnetic order, but strong spin fluctuations persist throughout the superconducting phase and are intimately linked to superconductivity. Neutron scattering measurements of spin fluctuations in hole-doped copper oxides have revealed an unusual 'hour-glass' feature in the momentum-resolved magnetic spectrum that is present in a wide range of superconducting and non-superconducting materials. There is no widely accepted explanation for this feature. One possibility is that it derives from a pattern of alternating spin and charge stripes, and this idea is supported by measurements on stripe-ordered La(1.875)Ba(0.125)CuO(4) (ref. 15). Many copper oxides without stripe order, however, also exhibit an hour-glass spectrum. Here we report the observation of an hour-glass magnetic spectrum in a hole-doped antiferromagnet from outside the family of superconducting copper oxides. Our system has stripe correlations and is an insulator, which means that its magnetic dynamics can conclusively be ascribed to stripes. The results provide compelling evidence that the hour-glass spectrum in the copper oxide superconductors arises from fluctuating stripes.

  1. Possible ground states and parallel magnetic-field-driven phase transitions of collinear antiferromagnets

    Science.gov (United States)

    Li, Hai-Feng

    2016-10-01

    Understanding the nature of all possible ground states and especially magnetic-field-driven phase transitions of antiferromagnets represents a major step towards unravelling the real nature of interesting phenomena such as superconductivity, multiferroicity or magnetoresistance in condensed-matter science. Here a consistent mean-field calculation endowed with antiferromagnetic (AFM) exchange interaction (J), easy axis anisotropy (γ), uniaxial single-ion anisotropy (D) and Zeeman coupling to a magnetic field parallel to the AFM easy axis consistently unifies the AFM state, spin-flop (SFO) and spin-flip transitions. We reveal some mathematically allowed exotic spin states and fluctuations depending on the relative coupling strength of (J, γ and D). We build the three-dimensional (J, γ and D) and two-dimensional (γ and D) phase diagrams clearly displaying the equilibrium phase conditions and discuss the origins of various magnetic states as well as their transitions in different couplings. Besides the traditional first-order type one, we unambiguously confirm an existence of a second-order type SFO transition. This study provides an integrated theoretical model for the magnetic states of collinear antiferromagnets with two interpenetrating sublattices and offers a practical approach as an alternative to the estimation of magnetic exchange parameters (J, γ and D), and the results may shed light on nontrivial magnetism-related properties of bulks, thin films and nanostructures of correlated electron systems.

  2. Polarized neutron powder diffraction studies of antiferromagnetic order in bulk and nanoparticle NiO

    DEFF Research Database (Denmark)

    Brok, Erik; Lefmann, Kim; Deen, Pascale P.;

    2015-01-01

    surface contribution to the magnetic anisotropy. Here we explore the potential use of polarized neutron diffraction to reveal the magnetic structure in NiO bulk and nanoparticle powders by applying the XYZ-polarization analysis method. Our investigations address in particular the spin orientation in bulk...... NiO and platelet-shaped NiO nanoparticles with thickness from greater than 200 nm down to 2.0 nm. The advantage of the applied method is that it is able to clearly separate the structural, the magnetic, and the spin-incoherent scattering signals for all particle sizes. For platelet-shaped particles......In many materials it remains a challenge to reveal the nature of magnetic correlations, including antiferromagnetism and spin disorder. Revealing the spin structure in magnetic nanoparticles is further complicated by the large incoherent neutron scattering cross section from water adsorbed...

  3. Measurement of Spin Correlation in Top Quark Pair Production at ATLAS

    CERN Document Server

    McLaughlan, Thomas

    2014-01-01

    This thesis presents a study of spin correlation in tt ̄ production in the ATLAS detector, in proton-proton collisions, corresponding to an integrated luminosity of 4.7 fb$^{−1}$, with a centre of mass energy of $\\sqrt{s}$ = 7 TeV. Both the dilepton and single lepton channels are considered, the latter providing a greater challenge due to the neccessity to reconstruct the down-type quark resulting from the W boson decay. A simple technique is employed to reconstruct single lepton $t\\bar{t}$ events, with the transverse angle between the charged lepton and down-type quark used as a probe of the spin correlation. In the dilepton channel, the transverse angle between both charged leptons is used. The extracted value of spin correlation in each channel is consistent with Standard Model predictions, with the result in the eμ channel alone sufficient to exclude a model without spin correlation at 7.8$\\sigma$. Also described is the author’s contribution to the maintenance and development of the Atlantis Event D...

  4. Correlation and disorder-enhanced nematic spin response in superconductors with weakly broken rotational symmetry

    DEFF Research Database (Denmark)

    Andersen, Brian Møller; Graser, S.; Hirschfeld, P. J.

    2012-01-01

    Recent experimental and theoretical studies have highlighted the possible role of an electronic nematic liquid in underdoped cuprate superconductors. We calculate, within a model of d-wave superconductor with Hubbard correlations, the spin susceptibility in the case of a small explicitly broken...

  5. Discrimination between spin-dependent charge transport and spin-dependent recombination in π-conjugated polymers by correlated current and electroluminescence-detected magnetic resonance

    Science.gov (United States)

    Kavand, Marzieh; Baird, Douglas; van Schooten, Kipp; Malissa, Hans; Lupton, John M.; Boehme, Christoph

    2016-08-01

    Spin-dependent processes play a crucial role in organic electronic devices. Spin coherence can give rise to spin mixing due to a number of processes such as hyperfine coupling, and leads to a range of magnetic field effects. However, it is not straightforward to differentiate between pure single-carrier spin-dependent transport processes which control the current and therefore the electroluminescence, and spin-dependent electron-hole recombination which determines the electroluminescence yield and in turn modulates the current. We therefore investigate the correlation between the dynamics of spin-dependent electric current and spin-dependent electroluminescence in two derivatives of the conjugated polymer poly(phenylene-vinylene) using simultaneously measured pulsed electrically detected (pEDMR) and optically detected (pODMR) magnetic resonance spectroscopy. This experimental approach requires careful analysis of the transient response functions under optical and electrical detection. At room temperature and under bipolar charge-carrier injection conditions, a correlation of the pEDMR and the pODMR signals is observed, consistent with the hypothesis that the recombination currents involve spin-dependent electronic transitions. This observation is inconsistent with the hypothesis that these signals are caused by spin-dependent charge-carrier transport. These results therefore provide no evidence that supports earlier claims that spin-dependent transport plays a role for room-temperature magnetoresistance effects. At low temperatures, however, the correlation between pEDMR and pODMR is weakened, demonstrating that more than one spin-dependent process influences the optoelectronic materials' properties. This conclusion is consistent with prior studies of half-field resonances that were attributed to spin-dependent triplet exciton recombination, which becomes significant at low temperatures when the triplet lifetime increases.

  6. Evolution of three-dimensional correlations during the photoinduced melting of antiferromagnetic order in La0.5Sr1.5MnO4

    NARCIS (Netherlands)

    Tobey, R. I.; Wall, S.; Foerst, M.; Bromberger, H.; Khanna, V.; Turner, J. J.; Schlotter, W.; Trigo, M.; Krupin, O.; Lee, W. S.; Chuang, Y. -D.; Moore, R.; Cavalieri, A. L.; Wilkins, S. B.; Zheng, H.; Mitchell, J. F.; Dhesi, S. S.; Cavalleri, A.; Hill, J.P.

    2012-01-01

    Using time-resolved resonant soft x-ray diffraction, we measure the evolution of the full three-dimensional scattering volume of the antiferromagnetic superlattice reflection in the single-layer manganite La0.5Sr1.5MnO4 on femtosecond time scales following photoexcitation. We find that the in-plane

  7. Quenched disorder and spin-glass correlations in XY nematics

    Energy Technology Data Exchange (ETDEWEB)

    Petridis, L; Terentjev, E M [Cavendish Laboratory, University of Cambridge, J J Thomson Avenue, Cambridge, CB3 0HE (United Kingdom)

    2006-08-04

    We present a theoretical study of the equilibrium ordering in a 3D XY nematic system with quenched random disorder. Within this model, treated with the replica trick and Gaussian variational method, the correlation length is obtained as a function of the local nematic order parameter Q and the effective disorder strength {gamma}. These results, {xi} {approx} Q{sup 2}e{sup 1/Q{sup 2}} and {xi} {approx} (1/{gamma}) e{sup -{gamma}}, clarify what happens in the limiting cases of diminishing Q and {gamma}, that is near a phase transition of a pure system. In particular, it is found that quenched disorder is irrelevant as Q {yields} 0 and hence does not change the character of the continuous XY nematic-isotropic phase transition. We discuss how these results compare with experiments and simulations.

  8. Magnetic structures of (Co{sub 2-x}Ni{sub x})(OH)PO{sub 4} (x = 0.1,0.3) spin glass-like state in antiferromagnetically ordered phases

    Energy Technology Data Exchange (ETDEWEB)

    Pedro, I de [Departamento de QuImica Inorganica, Facultad de Ciencia y TecnologIa, Universidad del PaIs Vasco, 48080 Bilbao (Spain); Rojo, J M [Departamento de QuImica Inorganica, Facultad de Ciencia y TecnologIa, Universidad del PaIs Vasco, 48080 Bilbao (Spain); Pizarro, J L [Departamento de MineralogIa y PetrologIa, Facultad de Ciencia y TecnologIa, Universidad del PaIs Vasco, 48080 Bilbao (Spain); Fernandez, J RodrIguez [CITIMAC, Facultad de Ciencias, Universidad de Cantabria, 39005 Santander (Spain); Marcos, J Sanchez [CITIMAC, Facultad de Ciencias, Universidad de Cantabria, 39005 Santander (Spain); Fernandez-DIaz, M T [Institut Laue-Langevin, BP 156X, F-38042 Grenoble Cedex (France); Arriortua, M I [Departamento de MineralogIa y PetrologIa, Facultad de Ciencia y TecnologIa, Universidad del PaIs Vasco, 48080 Bilbao (Spain); Rojo, T [Departamento de QuImica Inorganica, Facultad de Ciencia y TecnologIa, Universidad del PaIs Vasco, 48080 Bilbao (Spain)

    2006-04-19

    Compounds of the general formula Co{sub 2-x}Ni{sub x}(OH)PO{sub 4} (x = 0.1, 0.3) have been synthesized under mild hydrothermal conditions. Neutron powder diffraction, susceptibility and heat capacity measurements were carried out on polycrystalline samples. The cobalt-nickel compounds are ordered as three-dimensional antiferromagnets with ordering temperatures of 70 and 64 K for x = 0.1 and x = 0.3, respectively. The magnetic study shows a spin glass-like state below 11 and 5 K for Co{sub 1.9}Ni{sub 0.1}(OH)PO{sub 4} and Co{sub 1.7}Ni{sub 0.3}(OH)PO{sub 4}, respectively. Specific heat data present peaks at 68 and 61 K for Co{sub 1.9}Ni{sub 0.1} and Co{sub 1.7}Ni{sub 0.3}, respectively. These peaks show broad shoulders between approximately 15 and 40 K. The lack of any distinguishable anomaly below 10 K supports the spin glass nature of the low temperature transitions. Refinement of room temperature neutron diffraction data indicates that the Ni(II) ions are in octahedral co-ordination with the practical absence of these ions in the trigonal bipyramidal sites. The magnetic structures of Co{sub 2-x}Ni{sub x}(OH)PO{sub 4} consist of ferromagnetic arrangements between the octahedral chains and trigonal bipyramidal dimers within the xz plane with the magnetic moments along the z axis. The ferromagnetic layers are disposed antiparallel to one another along the y direction establishing the three-dimensional antiferromagnetic order (T{sub N}{approx}70 K for Co{sub 1.9}Ni{sub 0.1} and {approx}64 K for Co{sub 1.7}Ni{sub 0.3}). The different exchange pathways, the anisotropy of the Co(II) ions and the frustration of the magnetic moments in the trigonal bipyramidal geometry could be responsible for the freezing process.

  9. Mixing antiferromagnets to tune NiFe-[IrMn/FeMn] interfacial spin-glasses, grains thermal stability, and related exchange bias properties

    Energy Technology Data Exchange (ETDEWEB)

    Akmaldinov, K. [SPINTEC, UMR 8191 CNRS/INAC-CEA/UJF-Grenoble 1/Grenoble-INP, F-38054 Cedex (France); CROCUS Technology, F-38025 Grenoble (France); Ducruet, C.; Portemont, C. [CROCUS Technology, F-38025 Grenoble (France); Joumard, I.; Prejbeanu, I. L.; Dieny, B.; Baltz, V., E-mail: vincent.baltz@cea.fr [SPINTEC, UMR 8191 CNRS/INAC-CEA/UJF-Grenoble 1/Grenoble-INP, F-38054 Cedex (France)

    2014-05-07

    Spintronics devices and in particular thermally assisted magnetic random access memories require a wide range of ferromagnetic/antiferromagnetic (F/AF) exchange bias (EB) properties and subsequently of AF materials to fulfil diverse functionality requirements for the reference and storage. For the reference layer, large EB energies and high blocking temperature (T{sub B}) are required. In contrast, for the storage layer, mostly moderate T{sub B} are needed. One of the present issues is to find a storage layer with properties intermediate between those of IrMn and FeMn and in particular: (i) with a T{sub B} larger than FeMn for better stability at rest-T but lower than IrMn to reduce power consumption at write-T and (ii) with improved magnetic interfacial quality, i.e., with reduced interfacial glassy character for lower properties dispersions. To address this issue, the EB properties of F/AF based stacks were studied for various mixed [IrMn/FeMn] AFs. In addition to EB loop shifts, the F/AF magnetic interfacial qualities and the AF grains thermal stability are probed via measurements of the low- and high-temperature contributions to the T{sub B} distributions, respectively. A tuning of the above three parameters is observed when evolving from IrMn to FeMn via [IrMn/FeMn] repetitions.

  10. Magnetizing and heating quantum spin ladders

    Indian Academy of Sciences (India)

    Andrey Zheludev

    2008-11-01

    Quasi-one-dimensional quantum spin liquids, such as weakly coupled even-legged S=1/2 spin ladders or spin tubes, have a singlet non-magnetic ground state and gap in the excitation spectrum. Their low-temperature properties can be described in terms of triplet massive quasiparticles. These magnons possess some unique features due to the peculiar topology of one dimension. For example, two-particle interactions totally destroy single-particle states for certain energy and momentum transfers, resulting in the so-called termination of the magnon spectrum. At high field a Bose–Einstein condensation of these magnons produces a `quantum spin solid' phase, where `conventional` antiferromagnetic order coexists with excitations that are totally outside conventional spin wave theory. At finite temperatures strong repulsion between quasiparticles leads to a universal renormalization of their masses and lifetimes. These diverse phenomena are best probed by neutron scattering experiments that directly measure the spin correlation functions and excitation spectra.

  11. Emergent Power-Law Phase in the 2D Heisenberg Windmill Antiferromagnet: A Computational Experiment.

    Science.gov (United States)

    Jeevanesan, Bhilahari; Chandra, Premala; Coleman, Piers; Orth, Peter P

    2015-10-23

    In an extensive computational experiment, we test Polyakov's conjecture that under certain circumstances an isotropic Heisenberg model can develop algebraic spin correlations. We demonstrate the emergence of a multispin U(1) order parameter in a Heisenberg antiferromagnet on interpenetrating honeycomb and triangular lattices. The correlations of this relative phase angle are observed to decay algebraically at intermediate temperatures in an extended critical phase. Using finite-size scaling we show that both phase transitions are of the Berezinskii-Kosterlitz-Thouless type, and at lower temperatures we find long-range Z(6) order.

  12. Correlation functions of the half-infinite XXZ spin chain with a triangular boundary

    CERN Document Server

    Baseilhac, Pascal

    2014-01-01

    The half-infinite XXZ spin chain with a triangular boundary is considered in the massive regime. Two integral representations of correlation functions are proposed using bosonization. Sufficient conditions such that the expressions for triangular boundary conditions coincide with those for diagonal boundary conditions are identified. As an application, summation formulae of the boundary expectation values $\\langle \\sigma_1^a\\rangle $ with $a=z,\\pm$ are obtained. Exploiting the spin-reversal property, relations between $n$-fold integrals of elliptic theta functions are extracted.

  13. Quasi-one-dimensional spin-orbit-coupled correlated insulator in a multinuclear coordinated organometallic crystal

    Science.gov (United States)

    Merino, J.; Jacko, A. C.; Khosla, A. L.; Powell, B. J.

    2016-11-01

    We show how quasi-one-dimensional correlated insulating states arise at two-thirds filling in organometallic multinuclear coordination complexes described by layered decorated honeycomb lattices. The interplay of spin-orbit coupling and electronic correlations leads to pseudospin-one moments arranged in weakly coupled chains with highly anisotropic exchange and a large trigonal splitting. We show that the in-plane exchange coupling is very different from the interlayer coupling; in particular the latter is much larger, despite the underlying hopping integrals being close to isotropic. Surprisingly, the effective dimensionality of the pseudospin model is strongly dependent on the strength of the electronic correlations: With increasing Hubbard U the pseudospin-one model becomes increasingly one dimensional, even though the crystal is almost isotropic. We predict that the trigonal splitting leads to a quantum phase transition from a Haldane phase to a topologically trivial phase as the relative strength of the spin-orbit coupling increases.

  14. Configuration interaction combined with spin-projection for strongly correlated molecular electronic structures

    CERN Document Server

    Tsuchimochi, Takashi

    2015-01-01

    We introduce single and double particle-hole excitations in the recently revived spin-projected Hartree-Fock. Our motivation is to treat static correlation with spin-projection and recover the residual correlation, mostly dynamic in nature, with simple configuration interaction (CI). To this end, we introduce the Wick theorem for nonorhtogonal determinants, which enables an efficient implementation in conjunction with the direct CI scheme. The proposed approach, termed ECISD, achieves a balanced treatment between dynamic and static correlations. To approximately account for the quadruple excitations, we also modify the well-known Davidson correction. We report our approaches yield surprisingly accurate potential curves for HF, H2O, N2, and a hydrogen lattice, compared to traditional single reference wave function methods at the same computational scaling as regular CI.

  15. Effects of impurities and vortices on the low-energy spin excitations in high-Tc materials

    DEFF Research Database (Denmark)

    Andersen, Brian Møller; Graser, S.; Schmid, M.

    2011-01-01

    We review a theoretical scenario for the origin of the spin-glass phase of underdoped cuprate materials. In particular it is shown how disorder in a correlated d-wave superconductor generates a magnetic phase by inducing local droplets of antiferromagnetic order which eventually merge and form a ...... disorder and/or applied magnetic fields lead to a slowing down of the dynamical spin fluctuations in agreement with neutron scattering and muon spin rotation (mSR) experiments....

  16. Quantum phase transition between disordered and ordered states in the spin-1/2 kagome lattice antiferromagnet (Rb1-xCsx) 2Cu3SnF12

    Science.gov (United States)

    Katayama, Kazuya; Kurita, Nobuyuki; Tanaka, Hidekazu

    2015-06-01

    We have systematically investigated the variation of the exchange parameters and the ground state in the S =1/2 kagome-lattice antiferromagnet (Rb1 -xCsx )2Cu3SnF12 via magnetic measurements using single crystals. One of the parent compounds, Rb2Cu3SnF12 , which has a distorted kagome lattice accompanied by four sorts of nearest-neighbor exchange interaction, has a disordered ground state described by a pinwheel valence-bond-solid state. The other parent compound, Cs2Cu3SnF12 , which has a uniform kagome lattice at room temperature, has an ordered ground state with the q =0 spin structure. The analysis of magnetic susceptibilities shows that with increasing cesium concentration x , the exchange parameters increase with the tendency to be uniform. It was found that the ground state is disordered for x 0.53 . The pseudogap observed for x 0.53 approach zero at xc≃0.53 . This is indicative of the occurrence of a quantum phase transition at xc.

  17. Origin of Light-Induced Spin-Correlated Radical Pairs in Cryptochrome

    Science.gov (United States)

    Weber, Stefan; Biskup, Till; Okafuji, Asako; Marino, Anthony R.; Berthold, Thomas; Link, Gerhard; Hitomi, Kenichi; Getzoff, Elizabeth D.; Schleicher, Erik; Norris, James R.

    2012-01-01

    Blue-light excitation of cryptochromes and homologs uniformly triggers electron transfer (ET) from the protein surface to the flavin-adenine dinucleotide (FAD) cofactor. A cascade of three conserved tryptophan residues has been considered to be critically involved in this photoreaction. If the FAD is initially in its fully oxidized (diamagnetic) redox state, light-induced ET via the tryptophan triad generates a series of short-lived spin-correlated radical pairs comprising an FAD radical and a tryptophan radical. Coupled doublet-pair species of this type have been proposed as the basis, e.g., of a biological magnetic compass in migratory birds, and were found critical for some cryptochrome functions in vivo. In this contribution, a cryptochrome-like protein (CRYD) derived from Xenopus laevis has been examined as a representative system. The terminal radical-pair state FAD•⋯W324• of X. laevis CRYD has been characterized in detail by time-resolved electron-paramagnetic resonance (TREPR) at X-band microwave frequency (9.68 GHz) and magnetic fields around 345 mT, and at Q-band (34.08 GHz) at around 1215 mT. Different precursor states – singlet versus triplet – of radical-pair formation have been considered in spectral simulations of the experimental electron-spin polarized TREPR signals. Conclusively, we present evidence for a singlet-state precursor of FAD•⋯W324• radical-pair generation because at both magnetic fields, where radical pairs were studied by TREPR, net-zero electron-spin polarization has been detected. Neither a spin-polarized triplet precursor nor a triplet at thermal equilibrium can explain such an electron-spin polarization. It turns out that a two-microwave-frequency TREPR approach is essential to draw conclusions on the nature of the precursor electronic states in light-induced spin-correlated radical pair formations. PMID:20684534

  18. Magnetostructural correlations in the antiferromagnetic Co 2- x Cu x(OH)AsO 4 ( x=0 and 0.3) phases

    Science.gov (United States)

    de Pedro, I.; Rojo, J. M.; Pizarro, J. L.; Rodríguez Fernández, J.; Arriortua, M. I.; Rojo, T.

    2011-08-01

    The Co 2- xCu x(OH)AsO 4 ( x=0 and 0.3) compounds have been synthesized under mild hydrothermal conditions and characterized by X-ray single-crystal diffraction and spectroscopic data. The hydroxi-arsenate phases crystallize in the Pnnm orthorhombic space group with Z=4 and the unit-cell parameters are a=8.277(2) Å, b=8.559(2) Å, c=6.039(1) Å and a=8.316(1) Å, b=8.523(2) Å, c=6.047(1) Å for x=0 and 0.3, respectively. The crystal structure consists of a three-dimensional framework in which M(1)O 5-trigonal bipyramid dimers and M(2)O 6-octahedral chains ( M=Co and Cu) are present. Co 2(OH)AsO 4 shows an anomalous three-dimensional antiferromagnetic ordering influenced by the magnetic field below 21 K within the presence of a ferromagnetic component below the ordering temperature. When Co 2+ is partially substituted by Cu 2+ions, Co 1.7Cu 0.3(OH)AsO 4, the ferromagnetic component observed in Co 2(OH)AsO 4 disappears and the antiferromagnetic order is maintained in the entire temperature range. Heat capacity measurements show an unusual magnetic field dependence of the antiferromagnetic transitions. This λ-type anomaly associated to the three-dimensional antiferromagnetic ordering grows with the magnetic field and becomes better defined as observed in the non-substituted phase. These results are attributed to the presence of the unpaired electron in the d x2- y2 orbital and the absence of overlap between neighbour ions.

  19. Tailoring exchange couplings in magnetic topological-insulator/antiferromagnet heterostructures

    Science.gov (United States)

    He, Qing Lin; Kou, Xufeng; Grutter, Alexander J.; Yin, Gen; Pan, Lei; Che, Xiaoyu; Liu, Yuxiang; Nie, Tianxiao; Zhang, Bin; Disseler, Steven M.; Kirby, Brian J.; Ratcliff, William, II; Shao, Qiming; Murata, Koichi; Zhu, Xiaodan; Yu, Guoqiang; Fan, Yabin; Montazeri, Mohammad; Han, Xiaodong; Borchers, Julie A.; Wang, Kang L.

    2017-01-01

    Magnetic topological insulators such as Cr-doped (Bi,Sb)2Te3 provide a platform for the realization of versatile time-reversal symmetry-breaking physics. By constructing heterostructures exhibiting Néel order in an antiferromagnetic CrSb and ferromagnetic order in Cr-doped (Bi,Sb)2Te3, we realize emergent interfacial magnetic phenomena which can be tailored through artificial structural engineering. Through deliberate geometrical design of heterostructures and superlattices, we demonstrate the use of antiferromagnetic exchange coupling in manipulating the magnetic properties of magnetic topological insulators. Proximity effects are shown to induce an interfacial spin texture modulation and establish an effective long-range exchange coupling mediated by antiferromagnetism, which significantly enhances the magnetic ordering temperature in the superlattice. This work provides a new framework on integrating topological insulators with antiferromagnetic materials and unveils new avenues towards dissipationless topological antiferromagnetic spintronics.

  20. Evidence for Spin Correlation in t(t)over-bar Production

    Energy Technology Data Exchange (ETDEWEB)

    Abazov, V.M.; Abbott, B.; Acharya, B. S.; Adams, M.; Adams, T.; Alexeev, G. D.; Alkhazov, G.; Alton, A.; Alverson, G.; Alves, G. A.; Aoki, M.; Askew, A.; Asman, B.; Atkins, S.; Atramentov, O.; Augsten, K.; Avila, C.; BackusMayes, J.; Badaud, F.; Bagby, L.; Baldin, B.; Bandurin, D. V.; Banerjee, S.; Barberis, E.; Baringer, P.; Barreto, J.; Bartlett, J. F.; Bassler, U.; Bazterra, V.; Bean, A.; Begalli, M.; Belanger-Champagne, C.; Bellantoni, L.; Beri, S. B.; Bernardi, G.; Bernhard, R.; Bertram, I.; Besancon, M.; Beuselinck, R.; Bezzubov, V. A.; Bhat, P. C.; Bhatnagar, V.; Blazey, G.; Blessing, S.; Bloom, K.; Boehnlein, A.; Boline, D.; Boos, E. E.; Borissov, G.; Bose, T.; Brandt, A.; Brandt, O.; Brock, R.; Brooijmans, G.; Bross, A.; Brown, D.; Brown, J.; Bu, X. B.; Buehler, M.; Buescher, V.; Bunichev, V.; Burdin, S.; Burnett, T. H.; Buszello, C. P.; Calpas, B.; Camacho-Perez, E.; Carrasco-Lizarraga, M. A.; Casey, B. C. K.; Castilla-Valdez, H.; Chakrabarti, S.; Chakraborty, D.; Chan, K. M.; Chandra, A.; Chapon, E.; Chen, G.; Chevalier-Thery, S.; Cho, D. K.; Cho, S. W.; Choi, S.; Choudhary, B.; Cihangir, S.; Claes, D.; Clutter, J.; Cooke, M.; Cooper, W. E.; Corcoran, M.; Couderc, F.; Cousinou, M. -C.; Croc, A.; Cutts, D.; Das, A.; Davies, G.; De, K.; de Jong, S. J.; De la Cruz-Burelo, E.; Deliot, F.; Demina, R.; Denisov, D.; Denisov, S. P.; Desai, S.; Deterre, C.; DeVaughan, K.; Diehl, H. T.; Diesburg, M.; Ding, P. F.; Dominguez, A.; Dorland, T.; Dubey, A.; Dudko, L. V.; Duggan, D.; Duperrin, A.; Dutt, S.; Dyshkant, A.; Eads, M.; Edmunds, D.; Ellison, J.; Elvira, V. D.; Enari, Y.; Evans, H.; Evdokimov, A.; Evdokimov, V. N.; Facini, G.; Ferbel, T.; Fiedler, F.; Filthaut, F.; Fisher, W.; Fisk, H. E.; Fortner, M.; Fox, H.; Fuess, S.; Garcia-Bellido, A.; Garcia-Guerra, G. A.; Gavrilov, V.; Gay, P.; Geng, W.; Gerbaudo, D.; Gerber, C. E.; Gershtein, Y.; Ginther, G.; Golovanov, G.; Goussiou, A.; Grannis, P. D.; Greder, S.; Greenlee, H.; Greenwood, Z. D.; Gregores, E. M.; Grenier, G.; Gris, Ph; Grivaz, J. -F.; Grohsjean, A.; Gruenendahl, S.; Gruenewald, M. W.; Guillemin, T.; Gutierrez, G.; Gutierrez, P.; Haas, A.; Hagopian, S.; Haley, J.; Han, L.; Harder, K.; Harel, A.; Hauptman, J. M.; Hays, J.; Head, T.; Hebbeker, T.; Hedin, D.; Hegab, H.; Heinson, A. P.; Heintz, U.; Hensel, C.; la Cruz, I. Heredia-De; Herner, K.; Hesketh, G.; Hildreth, M. D.; Hirosky, R.; Hoang, T.; Hobbs, J. D.; Hoeneisen, B.; Hohlfeld, M.; Hubacek, Z.; Hynek, V.; Iashvili, I.; Ilchenko, Y.; Illingworth, R.; Ito, A. S.; Jabeen, S.; Jaffre, M.; Jamin, D.; Jayasinghe, A.; Jesik, R.; Johns, K.; Johnson, M.; Jonckheere, A.; Jonsson, P.; Joshi, J.; Jung, A. W.; Juste, A.; Kaadze, K.; Kajfasz, E.; Karmanov, D.; Kasper, P. A.; Katsanos, I.; Kehoe, R.; Kermiche, S.; Khalatyan, N.; Khanov, A.; Kharchilava, A.; Kharzheev, Y. N.; Kohli, J. M.; Kozelov, A. V.; Kraus, J.; Kulikov, S.; Kumar, A.; Kupco, A.; Kurca, T.; Kuzmin, V. A.; Kvita, J.; Lammers, S.; Landsberg, G.; Lebrun, P.; Lee, H. S.; Lee, S. W.; Lee, W. M.; Lellouch, J.; Li, L.; Li, Q. Z.; Lietti, S. M.; Lim, J. K.; Lincoln, D.; Linnemann, J.; Lipaev, V. V.; Lipton, R.; Liu, Y.; Lobodenko, A.; Lokajicek, M.; de Sa, R. Lopes; Lubatti, H. J.; Luna-Garcia, R.; Lyon, A. L.; Maciel, A. K. A.; Mackin, D.; Madar, R.; Magana-Villalba, R.; Malik, S.; Malyshev, V. L.; Maravin, Y.; Martinez-Ortega, J.; McCarthy, R.; McGivern, C. L.; Meijer, M. M.

    2012-01-19

    We present a measurement of the ratio of events with correlated t and {bar t} spins to the total number of t{bar t} events. This ratio f is evaluated using a matrix-element-based approach in 729 t{bar t} candidate events with a single lepton {ell} (electron or muon) and at least four jets. The analyzed p{bar p} collisions data correspond to an integrated luminosity of 5.3 fb{sup -1} and were collected with the D0 detector at the Fermilab Tevatron collider operating at a center-of-mass energy {radical}s = 1.96 TeV. Combining this result with a recent measurement of f in dileptonic final states, we find f in agreement with the standard model. In addition, the combination provides evidence for the presence of spin correlation in t{bar t} events with a significance of more than 3 standard deviations.

  1. S =1/2 triangular-lattice antiferromagnets Ba3CoSb2O9 and CsCuCl3: Role of spin-orbit coupling, crystalline electric field effect, and Dzyaloshinskii-Moriya interaction

    Science.gov (United States)

    Sera, A.; Kousaka, Y.; Akimitsu, J.; Sera, M.; Kawamata, T.; Koike, Y.; Inoue, K.

    2016-12-01

    We have performed the detailed investigations of the magnetization of the S =1/2 triangular-lattice antiferromagnets Ba3CoSb2O9 and CsCuCl3 with a 120∘ spin structure in the a b plane. In Ba3CoSb2O9 , the magnetic susceptibility (χ ) exhibits a broad maximum above the Néel temperature (TN) as is expected in the low-dimensional antiferromagnet (AFM). In CsCuCl3, χ exhibits a continuous increase down to TN as if it is the three-dimensional AFM. This is induced by the strong ferromagnetic (FM) interaction along the c axis. The magnetic phase diagrams are also very different. Although the transition field from the umbrella to the 2-1-coplanar phase (Hu -c) for H ∥c is almost independent of temperature in Ba3CoSb2O9 , it shows a considerable decrease with increasing temperature in CsCuCl3. The temperature independent Hu -c in Ba3CoSb2O9 originates from the magnetic anisotropy from the van Vleck contribution, which does not depend so much on the temperature. The temperature dependent Hu -c in CsCuCl3 originates from the magnetic anisotropy from the Dzyaloshinskii-Moriya (DM) interaction, which decreases with increasing temperature. For H ∥a b , the clear transition from the Y-coplanar to the up-up-down (u u d ) phase was observed in Ba3CoSb2O9 but not in CsCuCl3. While the reentrant behavior of TN originating from the thermal and quantum spin fluctuations is observed in both compounds, it is pronounced in Ba3CoSb2O9 but small in CsCuCl3. These differences originate from the existence or nonexistence of the DM interaction. The DM interaction in CsCuCl3 suppresses those fluctuations in the a b plane, leading to the less pronounced reentrant behavior of TN and the broad crossover in place of the phase transition. We analyzed the anisotropic magnetization of Ba3CoSb2O9 in the paramagnetic region by the mean field calculation. The spin-orbit (SO) coupling, the uniaxial crystalline electric field, and the isotropic exchange interaction were taken into account. We

  2. A Q-operator identity for the correlation functions of the infinite XXZ spin-chain

    Energy Technology Data Exchange (ETDEWEB)

    Korff, Christian [Centre for Mathematical Science, City University Northampton Square, London EC1V 0HB (United Kingdom)

    2005-07-29

    An explicit construction for Q-operators of the finite XXZ spin chain with twisted boundary conditions is presented. The massless and the massive regimes are considered as well as the root of unity case. It is explained how these results yield an alternative expression for the trace function employed in the description of the correlation functions of the inhomogeneous XXZ model on the infinite lattice by Boos, Jimbo, Miwa, Smirnov and Takeyama.

  3. Top Quark Pair Properties - Spin Correlation, Charge Asymmetry, and Complex Final States - at ATLAS

    Directory of Open Access Journals (Sweden)

    Brost Elizabeth

    2014-04-01

    Full Text Available We present measurements of top quark pair properties performed with the ATLAS detector at the Large Hadron Collider in proton-proton collisions at a center-of-mass energy of √s = 7 TeV. The latest measurements of spin correlation and charge asymmetry in tt¯$t\\overline t $ events, as well as measurements of the cross section for tt¯$t\\overline t $ production in association with vector bosons, are presented.

  4. Coexistence of antiferromagnetic and spin-glass behaviour in U{sub 3}Rh{sub 3}Sb{sub 4}

    Energy Technology Data Exchange (ETDEWEB)

    Tran, V H; Bukowski, Z; Stepien-Damm, J; Zaleski, A J; Badurski, D; Gorzelniak, R; Sulkowski, Cz; Troc, R [W Trzebiatowski Institute of Low Temperature and Structure Research, Polish Academy of Sciences, PO Box 1410, P-50-950 Wroclaw (Poland)

    2005-06-15

    We report on single-crystal growth, crystal structural determination and magnetic, electrical resistivity and thermoelectric power measurements performed on a set of single crystals of U{sub 3}Rh{sub 3}Sb{sub 4}. The compound crystallizes in the cubic Y{sub 3}Au{sub 3}Sb{sub 4}-type structure. The ac susceptibility and dc magnetization both indicate that the compound undergoes a transition into a spin-glass state below 14.7 K. The resistivity shows a broad minimum at 30 K. The thermoelectric power is negative in the whole temperature range studied and exhibits an enhanced value of -32 {mu}V K{sup -1} at room temperature.

  5. Double spin-glass-like behavior and antiferromagnetic superexchange interaction between Fe3+ ions in α-Ga2-xFexO3 (0 ≤ x ≤ 0.4)

    Science.gov (United States)

    Lv, Yi-Fei; Xiang, Jian-Yong; Wen, Fu-Sheng; Lv, Wei-Ming; Hu, Wen-Tao; Liu, Zhong-Yuan

    2015-03-01

    Single phase of Fe3+-doped α-Ga2-xFexO3 (α-GFxO, x = 0.1, 0.2, 0.3, 0.4) is synthesized by treating the β-Ga2-xFexO3 (β-GFxO) precursors at high temperatures and high pressures. Rietveld refinements of the X-ray diffraction data show that the lattice constants increase monotonically with the increase of Fe3+ content. Calorimetric measurements show that the temperature of the phase transition from α-GFxO to β-GFxO increases, while the associated enthalpy change decreases upon increasing Fe3+ content. The optical energy gap deduced from the reflectance measurement is found to decrease monotonically with the increase in Fe3+ content. From the measurements of magnetic field-dependent magnetization and temperature-dependent inverse molar susceptibility, we find that the superexchange interaction between Fe3+ ions is antiferromagnetic. Remnant magnetization is observed in the Fe3+-doped α-GFxO and is attributed to the spin glass in the magnetic sublattice. At high Fe3+ doping level (x = 0.4), two evident peaks are observed in the image part of the AC susceptibility . The frequency dependence in intensity of these two peaks as well as two spin freezing temperatures observed in the DC magnetization measurements of α-GF0.4O is suggested to be the behavior of two spin glasses. Project supported by the National Basic Research Program of China (Grant No. 2010CB731605), the National Science Fund for Distinguished Young Scholars of China (Grant No. 51025103), the National Natural Science Foundation of China (Grant Nos. 51172198 and 51102206), the Natural Science Foundation of Hebei Province, China (Grant No. E2014203144), the Science Foundation for the Excellent Youth Scholars from Universities and Colleges of Hebei Province, China (Grant No. YQ2014009), and the Research Program of the College Science & Technology of Hebei Province, China (Grant No. QN2014047).

  6. Spin-reorientation and weak ferromagnetism in antiferromagnetic TbMn{sub 0.5}Fe{sub 0.5}O{sub 3}

    Energy Technology Data Exchange (ETDEWEB)

    Nhalil, Hariharan, E-mail: hariharan@physics.iisc.ernet.in, E-mail: hariharan.nhalil@gmail.com; Sanathkumar, R.; Elizabeth, Suja [Department of Physics, Indian Institute of Science, Bangalore 560012 (India); Nair, Harikrishnan S. [Highly Correlated Matter Research Group, Physics Department, University of Johannesburg, P.O. Box 524, Auckland Park 2006 (South Africa); Strydom, André M. [Highly Correlated Matter Research Group, Physics Department, University of Johannesburg, P.O. Box 524, Auckland Park 2006 (South Africa); Max Planck Institute for Chemical Physics of Solids (MPICPfS), Nöthnitzerstraße 40, 01187 Dresden (Germany)

    2015-05-07

    Orthorhombic single crystals of TbMn{sub 0.5}Fe{sub 0.5}O{sub 3} are found to exhibit spin-reorientation, magnetization reversal, and weak ferromagnetism. Strong anisotropy effects are evident in the temperature dependent magnetization measurements along the three crystallographic axes a, b, and c. A broad magnetic transition is visible at T{sub N}{sup Fe/Mn}=286 K due to paramagnetic to A{sub x}G{sub y}C{sub z} ordering. A sharp transition is observed at T{sub SR}{sup Fe/Mn}=28 K, which is pronounced along c axis in the form of a sharp jump in magnetization where the spins reorient to G{sub x}A{sub y}F{sub z} configuration. The negative magnetization observed below T{sub SR}{sup Fe/Mn} along c axis is explained in terms of domain wall pinning. A component of weak ferromagnetism is observed in field-scans along c-axis but below 28 K. Field-induced steps-like transitions are observed in hysteresis measurement along b axis below 28 K. It is noted that no sign of Tb-order is discernible down to 2 K. TbMn{sub 0.5}Fe{sub 0.5}O{sub 3} could be highlighted as a potential candidate to evaluate its magneto-dielectric effects across the magnetic transitions.

  7. Immense Magnetic Response of Exciplex Light Emission due to Correlated Spin-Charge Dynamics

    Science.gov (United States)

    Wang, Yifei; Sahin-Tiras, Kevser; Harmon, Nicholas J.; Wohlgenannt, Markus; Flatté, Michael E.

    2016-01-01

    As carriers slowly move through a disordered energy landscape in organic semiconductors, tiny spatial variations in spin dynamics relieve spin blocking at transport bottlenecks or in the electron-hole recombination process that produces light. Large room-temperature magnetic-field effects (MFEs) ensue in the conductivity and luminescence. Sources of variable spin dynamics generate much larger MFEs if their spatial structure is correlated on the nanoscale with the energetic sites governing conductivity or luminescence such as in coevaporated organic blends within which the electron resides on one molecule and the hole on the other (an exciplex). Here, we show that exciplex recombination in blends exhibiting thermally activated delayed fluorescence produces MFEs in excess of 60% at room temperature. In addition, effects greater than 4000% can be achieved by tuning the device's current-voltage response curve by device conditioning. Both of these immense MFEs are the largest reported values for their device type at room temperature. Our theory traces this MFE and its unusual temperature dependence to changes in spin mixing between triplet exciplexes and light-emitting singlet exciplexes. In contrast, spin mixing of excitons is energetically suppressed, and thus spin mixing produces comparatively weaker MFEs in materials emitting light from excitons by affecting the precursor pairs. Demonstration of immense MFEs in common organic blends provides a flexible and inexpensive pathway towards magnetic functionality and field sensitivity in current organic devices without patterning the constituent materials on the nanoscale. Magnetic fields increase the power efficiency of unconditioned devices by 30% at room temperature, also showing that magnetic fields may increase the efficiency of the thermally activated delayed fluorescence process.

  8. Antiferromagnetic textures and dynamics on the surface of a heavy metal

    OpenAIRE

    Zarzuela, Ricardo; Tserkovnyak, Yaroslav

    2017-01-01

    We investigate the formation and dynamics of spin textures in antiferromagnetic insulators adjacent to a heavy-metal substrate with strong spin-orbit interactions. Exchange coupling to conduction electrons engenders an effective anisotropy, Dzyaloshinskii-Moriya interactions, and a magnetoelectric effect for the N\\'{e}el order, which can conspire to produce nontrivial antiferromagnetic textures. Current-driven spin transfer enabled by the heavy metal, furthermore, triggers ultrafast (THz) osc...

  9. Alignment correlation term in the {beta}-ray angular distribution from spin aligned {sup 20}Na

    Energy Technology Data Exchange (ETDEWEB)

    Minamisono, K. [TRIUMF, 4004 Wesbrook Mall, Vancouver, B. C., V6T 2A3 (Canada); Matsuta, K. [Department of Physics, Osaka University, Toyonaka 560-0043, Osaka (Japan); Minamisono, T. [Department of Physics, Osaka University, Toyonaka 560-0043, Osaka (Japan); Levy, C.D.P. [TRIUMF, 4004 Wesbrook Mall, Vancouver, B. C., V6T 2A3 (Canada); Nagatomo, T. [Department of Physics, Osaka University, Toyonaka 560-0043, Osaka (Japan); Ogura, M. [Department of Physics, Osaka University, Toyonaka 560-0043, Osaka (Japan); Sumikama, T. [Department of Physics, Osaka University, Toyonaka 560-0043, Osaka (Japan); Behr, J.A. [TRIUMF, 4004 Wesbrook Mall, Vancouver, B. C., V6T 2A3 (Canada); Jackson, K.P. [TRIUMF, 4004 Wesbrook Mall, Vancouver, B. C., V6T 2A3 (Canada); Fujiwara, H. [Department of Physics, Osaka University, Toyonaka 560-0043, Osaka (Japan); Mihara, M. [Department of Physics, Osaka University, Toyonaka 560-0043, Osaka (Japan); Fukuda, M. [Department of Physics, Osaka University, Toyonaka 560-0043, Osaka (Japan)

    2004-12-27

    The alignment correlation term in the {beta}-ray angular distribution from nuclear-spin aligned {sup 20}Na(I{sup {pi}} = 2{sup +}, T{sub 1/2} = 449.7 ms) has been measured for the first time. A large enhancement of the time component d in the main axial vector current was preliminarily obtained and the higher order matrices j{sub 2} and j{sub 3} were also evaluated. In order to extract very small G-parity violating induced tensor term, the alignment correlation term of the mirror partner {sup 20}F have to be measured.

  10. Correlated calculations of indirect nuclear spin-spin coupling constants using second-order polarization propagator approximations: SOPPA and SOPPA(CCSD)

    DEFF Research Database (Denmark)

    Enevoldsen, Thomas; Oddershede, Jens; Sauer, Stephan P. A.

    1998-01-01

    We present correlated calculations of the indirect nuclear spin-spin coupling constants of HD, HF, H2O, CH4, C2H2, BH, AlH, CO and N2 at the level of the second-order polarization propagator approximation (SOPPA) and the second-order polarization propagator approximation with coupled-cluster sing......We present correlated calculations of the indirect nuclear spin-spin coupling constants of HD, HF, H2O, CH4, C2H2, BH, AlH, CO and N2 at the level of the second-order polarization propagator approximation (SOPPA) and the second-order polarization propagator approximation with coupled......-cluster singles and doubles amplitudes - SOPPA(CCSD). Attention is given to the effect of the so-called W 4 term, which has not been included in previous SOPPA spin-spin coupling constant studies of these molecules. Large sets of Gaussian basis functions, optimized for the calculation of indirect nuclear spin...

  11. Quasiparticle band structure of antiferromagnetic Eu Te

    Energy Technology Data Exchange (ETDEWEB)

    Mathi Jaya, S.; Nolting, W. [Humboldt-Universitaet zu Berlin, Institut fuer Physik, Lehrstuhl Festkoerpertheorie, Invalidenstrasse 110, D-10115 Berlin (Germany)

    1997-11-24

    The temperature-dependent electronic quasiparticle spectrum of the antiferromagnetic semiconductor Eu Te is derived by use of a combination of a many-body model procedure with a tight-binding-'linear muffin tin orbital' (TB - LMTO) band structure calculation. The central part is the d-f model for a single band electron ('test electron') being exchange coupled to the anti ferromagnetically ordered localized moments of the Eu ions. The single-electron Bloch energies of the d-f model are taken from a TB-LMTO calculation for paramagnetic Eu Te. The d-f model is evaluated by a recently proposed moment conserving Green function technique to get the temperature-dependent sublattice-quasiparticle band structure (S-QBS) and sublattice-quasiparticle density of states (S-QDOS) of the unoccupied 5 d-6 s energy bands. Unconventional correlation effects and the appearance of characteristic quasiparticles ('magnetic polarons') are worked out in detail. The temperature dependence of the S-QDOS and S-QBS is mainly provoked by the spectral weights of the energy dispersions. Minority- and majority-spin spectra coincide for all temperatures but with different densities of states. Upon cooling from T{sub N} to T = 0 K the lower conduction band edge exhibits a small blue shift of -0.025 eV in accordance with the experiment. Quasiparticle damping manifesting itself in a temperature-dependent broadening of the spectral density peaks arises from spin exchange processes between (5 d-6 s) conduction band electrons and localized 4 f moments. (author)

  12. Quantum Phase Transitions in Anti-ferromagnetic Planar Cubic Lattices

    CERN Document Server

    Wellard, C J; Wellard, Cameron; Orus, Roman

    2004-01-01

    Motivated by its relation to an NP-hard problem we analyze the ground state properties of anti-ferromagnetic Ising-spin networks in planar cubic lattices under the action of homogeneous transverse and longitudinal magnetic fields. We consider different instances of the cubic geometry and find a set of quantum phase transitions for each one of the systems, which we characterize by means of entanglement behavior and majorization theory. Entanglement scaling at the critical region is in agreement with results arising from conformal symmetry, therefore even the simplest planar systems can display very large amounts of quantum correlation. No conclusion can be made as to the scaling behavior of the minimum energy gap, with the data allowing equally good fits to exponential and power law decays. Analysis of entanglement and especially of majorization instead of the energy spectrum proves to be a good way of detecting quantum phase transitions in highly frustrated configurations.

  13. Classical and quantum anisotropic Heisenberg antiferromagnets

    Directory of Open Access Journals (Sweden)

    W. Selke

    2009-01-01

    Full Text Available We study classical and quantum Heisenberg antiferromagnets with exchange anisotropy of XXZ-type and crystal field single-ion terms of quadratic and quartic form in a field. The magnets display a variety of phases, including the spin-flop (or, in the quantum case, spin-liquid and biconical (corresponding, in the quantum lattice gas description, to supersolid phases. Applying ground-state considerations, Monte Carlo and density matrix renormalization group methods, the impact of quantum effects and lattice dimension is analysed. Interesting critical and multicritical behaviour may occur at quantum and thermal phase transitions.

  14. Investigation of spin correlations in top-pair production with the CMS detector at the LHC

    Energy Technology Data Exchange (ETDEWEB)

    Davids, Martina

    2011-02-25

    In spring 2010 the Large Hadron Collider (LHC) started its operation with a center-of-mass energy of 7 TeV, that will be increased up to 14 TeV in the following years. Considering a medium energy of {radical}(s)=10 TeV and a luminosity of L=10{sup 33} cm{sup -2}s{sup -1} some million top quarks are produced per year. This offers the opportunity to investigate spin-correlations between the top quarks from pair production. As the spinconfiguration of the top-quark pair depends on the production mechanism, a measurement of such effects is a unique tool to study the contributions of the production processes and spin effects. This allows to test the Standard Model. This thesis investigates dileptonic top-pair decays at the Compact Muon Solenoid based on simulated events. A quantitative measure of spin correlations is the asymmetry A, that manifests itself in the angular distribution of the two leptons. A full kinematic reconstruction of the top pair is necessary to determine this distribution. The MC generators Pythia, MC rate at NLO, and TopReX are tested with respect to their treatment of spin-correlations. Pythia is used to generate uncorrelated samples. MC rate at NLO reproduces the Standard Model prediction. These samples are used to determine the sensitivity of the present analysis. Due to an incorrect implementation of the helicity states, TopReX is not usable. A full event selection and reconstruction are adapted. The reconstructed angular distribution shows a significant distortion. A template method is implemented to determine the asymmetry. Here, the angular distribution is decomposed into a flat, a completely asymmetric, and a background part, that are fitted by a binned {chi}{sup 2} approach to toy-data. An ensemble study is performed to estimate the statistical uncertainty. As the main systematic uncertainties, generator effects, the jet energy scale and uncertainties in the cross sections or selection efficiency are investigated. Considering an integrated

  15. Correlation-Driven Charge and Spin Fluctuations in LaCoO3

    Science.gov (United States)

    Karolak, M.; Izquierdo, M.; Molodtsov, S. L.; Lichtenstein, A. I.

    2015-07-01

    The spin transition in LaCoO3 has been investigated using density-functional theory in combination with dynamical mean-field theory employing continuous time quantum Monte Carlo and exact diagonalization impurity solvers. Calculations on the experimental rhombohedral atomic structure with two Co sites per unit cell show that an independent treatment of the Co atoms results in a ground state with strong charge fluctuations induced by electronic correlations. Each atom shows a contribution from either a d5 or a d7 state in addition to the main d6 state. These states play a relevant role in the spin transition which can be understood as a low spin-high spin (LS-HS) transition with significant contributions (˜10 % ) to the LS and HS states of d5 and d7 states, respectively. We report spectra as well as optical conductivity data for all cases. A thermodynamic analysis reveals a significant kinetic energy gain through introduction of charge fluctuations, which in addition to the potential energy reduction lowers the total energy of the system.

  16. Theoretical investigation on the relationship between the torque correlation and spin correlation models for the Gilbert damping constant

    Science.gov (United States)

    Sakuma, Akimasa

    2015-01-01

    To gain insight into the relationship between the spin correlation (SC) and torque correlation (TC) models for the Gilbert damping constant, α, we first make a simple consideration on the physical aspect of these models and calculate α for the Fe50Co50 disordered alloy by the two models using the first principles technique. Electron scattering is introduced through the random arrangement of atoms and is treated with coherent potential approximation. The results indicate that in the TC model, vertex correction (VC) does not have significant contribution and the results are insensitive to the infinitesimal positive value, δ, which is used in Green's function. In the SC model, on the other hand, the VC is indispensable and the obtained values of α are found to be considerably sensitive to δ. We confirm that the value of α in the SC model approaches the value obtained in the TC model in the limit δ→+0 .

  17. Polyakov loop and spin correlators on finite lattices a study beyond the mass gap

    CERN Document Server

    Engels, J; Neuhaus, T; Engels, J; Mitrjushkin, V K; Neuhaus, T

    1995-01-01

    We derive an analytic expression for point-to-point correlation functions of the Polyakov loop based on the transfer matrix formalism. For the 2d Ising model we show that the results deduced from point-point spin correlators are coinciding with those from zero momentum correlators. We investigate the contributions from eigenvalues of the transfer matrix beyond the mass gap and discuss the limitations and possibilities of such an analysis. The finite size behaviour of the obtained 2d Ising model matrix elements is examined. The point-to-point correlator formula is then applied to Polyakov loop data in finite temperature SU(2) gauge theory. The leading matrix element shows all expected scaling properties. Just above the critical point we find a Debye screening mass ~\\mu_D/T\\approx4~, independent of the volume.

  18. Spins, Stripes, and Superconductivity in Hole-Doped Cuprates

    OpenAIRE

    Tranquada, John M.

    2013-01-01

    One of the major themes in correlated electron physics over the last quarter century has been the problem of high-temperature superconductivity in hole-doped copper-oxide compounds. Fundamental to this problem is the competition between antiferromagnetic spin correlations, a symptom of strong Coulomb interactions, and the kinetic energy of the doped carriers, which favors delocalization. After discussing some of the early challenges in the field, I describe the experimental picture provided b...

  19. A Kagome Map of Spin Liquidsx

    Science.gov (United States)

    Essafi, Karim; Benton, Owen; Jaubert, Ludovic D. C.

    Competing interactions in frustrated magnets prevent ordering down to very low temperatures and stabilize exotic highly degenerate phases where strong correlations coexist with fluctuations. We study a very general nearest-neighbour Heisenberg spin model Hamiltonian on the kagome lattice which consist of Dzyaloshinskii-Moriya, ferro- and antiferromagnetic interactions. We present a three-fold mapping which transforms the well-known Heisenberg antiferromagnet (HAF) and XXZ model onto two lines of time-reversal Hamiltonians. The mapping is exact for both classical and quantum spins, i.e. preserves the energy spectrums of the HAF and XXZ model. As a consequence, our three-fold mapping gives rise to a connected network of quantum spin liquids centered around the Ising antiferromagnet. We show that this quantum disorder spreads over an extended region of the phase diagram at linear order in spin wave theory, which overlaps with the parameter region of Herbertsmithite ZnCu3(OH)6Cl2. At the classical level, all the phases have an extensively degenerate ground-state which present a variety of properties such as ferromagnetically induced pinch points in the structure factor and spontaneous scalar chirality which was absent in the original HAF and XXZ models. This work was supported by the Okinawa Institute of Science and Technology Graduate University.

  20. Macroscopic anisotropy and symmetry breaking in the pyrochlore antiferromagnet Gd2Ti2O7

    Science.gov (United States)

    Hassan, A. K.; Lévy, L. P.; Darie, C.; Strobel, P.

    2003-06-01

    In the Heisenberg antiferromagnet Gd2Ti2O7, the exchange interactions are geometrically frustrated by the pyrochlore lattice structure. This ESR study reveals a strong temperature dependent anisotropy with respect to a [111] body diagonal below a temperature TA=80 K, despite the spin only nature of the Gd3+ ion. Anisotropy and symmetry breaking can nevertheless appear through the superexchange interaction. In the presence of anisotropic exchanges, short range planar correlations restricted to specific Kagomé planes are sufficient to explain the two ESR modes studied in this work.

  1. Large off-diagonal magnetoelectric coupling in the quantum paraelectric antiferromagnet EuTiO3

    Science.gov (United States)

    Shvartsman, V. V.; Borisov, P.; Kleemann, W.; Kamba, S.; Katsufuji, T.

    2010-02-01

    The third-order E2H2 -type magnetoelectric (ME) response of polycrystalline EuTiO3 changes sign under magnetic bias and shows a large anomaly at the antiferromagnetic (AF)-paramagnetic phase boundary below TN≈5.3K . It is attributed to critical fluctuations of the AF order parameter reinforced by quantum paraelectric polar correlations. The underlying biquadratic spin-lattice coupling involves electric field induced Dzyaloshinskii-Moriya interaction as described within mean-field approximation. Single domaining by ME annealing (or cooling) significantly enhances the response by additional EH and EH2 effects.

  2. Finite-size scaling effect on Néel temperature of antiferromagnetic Cr2O3 (0001) films in exchange-coupled heterostructures

    Science.gov (United States)

    Pati, Satya Prakash; Al-Mahdawi, Muftah; Ye, Shujun; Shiokawa, Yohei; Nozaki, Tomohiro; Sahashi, Masashi

    2016-12-01

    The scaling of antiferromagnetic ordering temperature of corundum-type chromia films has been investigated. Néel temperature TN was determined from the effect of perpendicular exchange bias on the magnetization of a weakly-coupled adjacent ferromagnet. For a thick-film case, the validity of detection is confirmed by a susceptibility measurement. Detection of TN was possible down to 1-nm-thin chromia films. The scaling of ordering temperature with thickness was studied using different buffering materials and compared with Monte-Carlo simulations. The spin-correlation length and the corresponding critical exponent were estimated, and they were consistent between experimental and simulation results. The spin-correlation length is an order of magnitude less than cubic antiferromagnets. We propose that the difference is from the change of number of exchange-coupling links in the two crystal systems.

  3. Computational Electronic Structure of Antiferromagnetic Centers in Metalloproteins.

    Science.gov (United States)

    Rodriguez, Jorge H.

    2003-03-01

    Nature uses the properties of transition metal ions to carry out a variety of functions associated with vital life processes such as respiration and the transport of oxygen. Oxo-bridged diiron centers are intriguing structural motifs which are present in dioxygen transporting proteins and display antiferromagnetic ordering. We have performed a comprehensive study of the electronic structure and magnetic properties of structurally characterized models for diiron-oxo proteins. Results from Kohn-Sham density functional theory show that the models are antiferromagnetically coupled in agreement with experiment. The physical origin of the spin coupling has been elucidated as the main superexchange pathways responsible for magnetic ordering have been identified. In addition, the exchange constants that parameterize the Heisenberg Hamiltonian, H=JS_1.S_2, have been predicted in excellent agreement with experiment. Our results are important for establishing correlations between electronic structure and biomolecular function and show that computational electronic structure can be used as a powerful tool for the investigation of biomolecular magnetism.

  4. Spin-orbit and electron correlation effects on the structure of EF3 (E = I, At, and element 117).

    Science.gov (United States)

    Kim, Hyoseok; Choi, Yoon Jeong; Lee, Yoon Sup

    2008-12-18

    Structures and vibrational frequencies of group 17 fluorides EF3 (E = I, At, and element 117) are calculated at the density functional theory (DFT) level of theory using relativistic effective core potentials (RECPs) with and without spin-orbit terms in order to investigate the effects of spin-orbit interactions and electron correlations on the structures and vibrational frequencies of EF3. Various tests imply that spin-orbit and electron correlation effects estimated presently from Hartree-Fock (HF) and DFT calculations with RECPs with and without spin-orbit terms are quite reasonable. Spin-orbit and electron correlation effects generally increase bond lengths and/or angles in both C2v and D3h structures. For IF3, the C2v structure is a global minimum, and the D3h structure is a second-order saddle point in both HF and DFT calculations with and without spin-orbit interactions. Spin-orbit effects for IF3 are negligible in comparison to electron correlation effects. The D3h global minimum is the only minimum structure for (117)F3 in all RECP calculations, and the C2v structure is neither a local minimum nor a saddle point. In the case of AtF3, the C2v structure is found to be a local minimum in all RECP calculations without spin-orbit terms, and the D3h structure becomes a local minimum at the DFT level of theory with and without spin-orbit interactions. In the HF calculation with spin-orbit terms, the D3h structure of AtF3 is a second-order saddle point. AtF3 is a borderline case between the valence-shell-electron-pair-repulsion (VSEPR) structure of IF3 and the non-VSEPR structure of (117)F3. Relativistic effects, including scalar relativistic and spin-orbit effects, and electron correlation effects together or separately stabilize the D3h structures more than the C2v structures. As a result, one may suggest that the VSEPR predictions agree very well with the structures optimized by the nonrelativistic HF level of theory even for heavy-atom molecules but not so

  5. Scaled Opposite Spin Second Order Moller-Plesset Correlation Energy: An Economical Electronic Structure Method

    Energy Technology Data Exchange (ETDEWEB)

    Jung, Yousung; Lochan, Rohini C.; Dutoi, Anthony D.; Head-Gordon, Martin

    2004-08-02

    A simplified approach to treating the electron correlation energy is suggested in which only the alpha-beta component of the second order Moller-Plesset energy is evaluated, and then scaled by an empirical factor which is suggested to be 1.3. This scaled opposite spin second order energy (SOS-MP2) yields results for relative energies and derivative properties that are statistically improved over the conventional MP2 method. Furthermore, the SOS-MP2 energy can be evaluated without the 5th order computational steps associated with MP2 theory, even without exploiting any spatial locality. A 4th order algorithm is given for evaluating the opposite spin MP2 energy using auxiliary basis expansions, and a Laplace approach, and timing comparisons are given.

  6. Charge dynamics of the antiferromagnetically ordered Mott insulator

    Science.gov (United States)

    Han, Xing-Jie; Liu, Yu; Liu, Zhi-Yuan; Li, Xin; Chen, Jing; Liao, Hai-Jun; Xie, Zhi-Yuan; Normand, B.; Xiang, Tao

    2016-10-01

    We introduce a slave-fermion formulation in which to study the charge dynamics of the half-filled Hubbard model on the square lattice. In this description, the charge degrees of freedom are represented by fermionic holons and doublons and the Mott-insulating characteristics of the ground state are the consequence of holon-doublon bound-state formation. The bosonic spin degrees of freedom are described by the antiferromagnetic Heisenberg model, yielding long-ranged (Néel) magnetic order at zero temperature. Within this framework and in the self-consistent Born approximation, we perform systematic calculations of the average double occupancy, the electronic density of states, the spectral function and the optical conductivity. Qualitatively, our method reproduces the lower and upper Hubbard bands, the spectral-weight transfer into a coherent quasiparticle band at their lower edges and the renormalisation of the Mott gap, which is associated with holon-doublon binding, due to the interactions of both quasiparticle species with the magnons. The zeros of the Green function at the chemical potential give the Luttinger volume, the poles of the self-energy reflect the underlying quasiparticle dispersion with a spin-renormalised hopping parameter and the optical gap is directly related to the Mott gap. Quantitatively, the square-lattice Hubbard model is one of the best-characterised problems in correlated condensed matter and many numerical calculations, all with different strengths and weaknesses, exist with which to benchmark our approach. From the semi-quantitative accuracy of our results for all but the weakest interaction strengths, we conclude that a self-consistent treatment of the spin-fluctuation effects on the charge degrees of freedom captures all the essential physics of the antiferromagnetic Mott-Hubbard insulator. We remark in addition that an analytical approximation with these properties serves a vital function in developing a full understanding of the

  7. Enhanced exchange anisotropy in IrMn/CoFeB systems and its correlation with uncompensated interfacial spins

    DEFF Research Database (Denmark)

    Du, Yuqing; Pan, Genhua; Moate, Roy;

    2010-01-01

    Bottom pinned exchange bias systems of IrMn/CoFe and IrMn/CoFeB on CoFe seed layers were studied. Enhanced exchange anisotropy has been observed for IrMn/CoFeB samples annealed at 350 °C. The ferromagnetic and antiferromagnetic layers of both samples are polycrystalline and textured {110} for the......Bottom pinned exchange bias systems of IrMn/CoFe and IrMn/CoFeB on CoFe seed layers were studied. Enhanced exchange anisotropy has been observed for IrMn/CoFeB samples annealed at 350 °C. The ferromagnetic and antiferromagnetic layers of both samples are polycrystalline and textured {110......} for the CoFe and CoFeB, and {111} for IrMn. Results demonstrated that the enhanced exchange anisotropy in the IrMn/CoFeB system is closely associated with the increased uncompensated interfacial spins as evidenced by the enhanced Mn x-ray magnetic circular dichroism (XMCD) signal strength. A quantitative...

  8. Translationally invariant treatment of pair correlations in nuclei; 1, spin and isospin dependent correlations

    CERN Document Server

    Guardiola, R; Navarro, J; Bishop, R F; Puente, A; Walet, N R; Walet, Niels R.

    1996-01-01

    We study the extension of our translationally invariant treatment of few-body nuclear systems to heavier nuclei. At the same time we also introduce state-dependent correlation operators. Our techniques are tailored to those nuclei that can be dealt with in $LS$ coupling, which includes all nuclei up to the shell closure at $A=40$. We study mainly $p$-shell nuclei in this paper. A detailed comparison with other microscopic many-body approaches is made, using a variety of schematic nuclear interactions. It is shown that our methodology produces very good energies, and presumably also wave functions, for medium mass nuclei.

  9. Pairwise correlations via quantum discord and its geometric measure in a four-qubit spin chain

    Directory of Open Access Journals (Sweden)

    Abdel-Baset A. Mohamed

    2013-04-01

    Full Text Available The dynamic of pairwise correlations, including quantum entanglement (QE and discord (QD with geometric measure of quantum discord (GMQD, are shown in the four-qubit Heisenberg XX spin chain. The results show that the effect of the entanglement degree of the initial state on the pairwise correlations is stronger for alternate qubits than it is for nearest-neighbor qubits. This parameter results in sudden death for QE, but it cannot do so for QD and GMQD. With different values for this entanglement parameter of the initial state, QD and GMQD differ and are sensitive for any change in this parameter. It is found that GMQD is more robust than both QD and QE to describe correlations with nonzero values, which offers a valuable resource for quantum computation.

  10. The role of three-gluon correlation functions in the single spin asymmetry

    Directory of Open Access Journals (Sweden)

    Beppu Hiroo

    2015-01-01

    Full Text Available We study the twist-3 three-gluon contribution to the single spin asymmetry in the light-hadron production in pp collision in the framework of the collinear factorization. We derive the corresponding cross section formula in the leading order with respect to the QCD coupling constant. We also present a numerical calculation of the asymmetry at the RHIC energy, using a model for the three-gluon correlation functions suggested by the asymmetry for the D-meson production at RHIC. We found that the asymmetries for the light-hadron and the jet productions are very useful to constrain the magnitude and form of the correlation functions. Since the three-gluon correlation functions shift the asymmetry for all kinds of hadrons in the same direction, it is unlikely that they become a main source of the asymmetry.

  11. Mn2Au: body-centered-tetragonal bimetallic antiferromagnets grown by molecular beam epitaxy.

    Science.gov (United States)

    Wu, Han-Chun; Liao, Zhi-Min; Sofin, R G Sumesh; Feng, Gen; Ma, Xiu-Mei; Shick, Alexander B; Mryasov, Oleg N; Shvets, Igor V

    2012-12-11

    Mn(2)Au, a layered bimetal, is successfully grown using molecular beam epitaxy (MBE). The experiments and theoretical calculations presented suggest that Mn(2)Au film is antiferromagnetic with a very low critical temperature. The antiferromagnetic nature is demonstrated by measuring the exchange-bias effect of Mn(2)Au/Fe bilayers. This study establishes a primary basis for further research of this new antiferromagnet in spin-electronic device applications.

  12. Quantum correlation dynamics subjected to critical spin environment with short-range anisotropic interaction

    Science.gov (United States)

    Guo, J. L.; Zhang, X. Z.

    2016-01-01

    Short-range interaction among the spins can not only results in the rich phase diagram but also brings about fascinating phenomenon both in the contexts of quantum computing and information. In this paper, we investigate the quantum correlation of the system coupled to a surrounding environment with short-range anisotropic interaction. It is shown that the decay of quantum correlation of the central spins measured by pairwise entanglement and quantum discord can serve as a signature of quantum phase transition. In addition, we study the decoherence factor of the system when the environment is in the vicinity of the phase transition point. In the strong coupling regime, the decay of the decoherence factor exhibits Gaussian envelop in the time domain. However, in weak coupling limit, the quantum correlation of the system is robust against the disturbance of the magnetic field through optimal control of the anisotropic short-range interaction strength. Based on this, the effects of the short-range anisotropic interaction on the sudden transition from classical to quantum decoherence are also presented. PMID:27596050

  13. Two-dimensional MAS NMR correlation protocols involving double-quantum filtering of quadrupolar spin-pairs.

    Science.gov (United States)

    Edén, Mattias

    2010-05-01

    Three two-dimensional (2D) NMR homonuclear correlation techniques invoking double-quantum (2Q) filtration of the central transitions of half-integer spins are evaluated numerically and experimentally. They correlate directly detected single-quantum (1Q) coherences in the t(2) domain with either of 1Q, two-spin 2Q or single-spin multiple-quantum coherence-evolutions in the indirect (t(1)) dimension. We employ experimental (23)Na and (27)Al NMR on sodium sulfite and the natural mineral sillimanite (SiAl(2)O(5)), in conjunction with simulated 2D spectra from pairs of dipolar-recoupled spins-3/2 and 5/2 at different external magnetic fields, to compare the correlation strategies from the viewpoints of 2D spectral resolution, signal sensitivity, implementational aspects and their relative merits for establishing internuclear proximities and quadrupolar tensor orientations.

  14. Top quark pair properties: spin correlation, charge asymmetry and complex final states at LHC in ATLAS

    Directory of Open Access Journals (Sweden)

    Rubbo Francesco

    2013-11-01

    Full Text Available In proton–proton collisions at the LHC, pairs of top and anti-top quarks are expected to be mostly produced through gluon fusion, in contrast to production at the Tevatron, where quark annihilation dominates. Making use of the large number of top quark pairs, we present measurements of the spin correlation between top and anti-top quarks as well as of the top quark charge asymmetry, which constitute important tests of QCD and are sensitive to new physics. We also discuss top production in association of photons and Z bosons.

  15. Thermal Phase Transitions of Strongly Correlated Bosons with Spin-Orbit Coupling

    Science.gov (United States)

    Hickey, Ciarán; Paramekanti, Arun

    2014-12-01

    Experiments on ultracold atoms have started to explore lattice effects and thermal fluctuations for two-component bosons with spin-orbit coupling (SOC). Motivated by this, we derive and study a t J model for lattice bosons with equal Rashba-Dresselhaus SOC and strong Hubbard repulsion in a uniform Zeeman magnetic field. Using the Gutzwiller ansatz, we find strongly correlated ground states with stripe superfluid (SF) order. We formulate a finite temperature generalization of the Gutzwiller method, and show that thermal fluctuations in the doped Mott insulator drive a two-step melting of the stripe SF, revealing a wide regime of a stripe normal fluid.

  16. Spins, stripes, and superconductivity in hole-doped cuprates

    Science.gov (United States)

    Tranquada, John M.

    2013-08-01

    One of the major themes in correlated electron physics over the last quarter century has been the problem of high-temperature superconductivity in hole-doped copper-oxide compounds. Fundamental to this problem is the competition between antiferromagnetic spin correlations, a symptom of strong Coulomb interactions, and the kinetic energy of the doped carriers, which favors delocalization. After discussing some of the early challenges in the field, I describe the experimental picture provided by a variety of spectroscopic and transport techniques. Then I turn to the technique of neutron scattering, and discuss how it is used to determine spin correlations, especially in model systems of quantum magnetism. Neutron scattering and complementary techniques have determined the extent to which antiferromagnetic spin correlations survive in the cuprate superconductors. One experimental case involves the ordering of spin and charge stripes. I first consider related measurements on model compounds, such as La2-xSrxNiO4+δ, and then discuss the case of La2-xBaxCuO4. In the latter system, recent transport studies have demonstrated that quasi-two-dimensional superconductivity coexists with the stripe order, but with frustrated phase order between the layers. This has led to new concepts for the coexistence of spin order and superconductivity. While the relevance of stripe correlations to high-temperature superconductivity remains a subject of controversy, there is no question that stripes are an intriguing example of electron matter that results from strong correlations.

  17. Magnetic field sensing subject to correlated noise with a ring spin chain

    Science.gov (United States)

    Guo, Li-Sha; Xu, Bao-Ming; Zou, Jian; Shao, Bin

    2016-09-01

    In this paper, we focus on the magnetic field sensing subject to a correlated noise. We use a ring spin chain with only the nearest neighbor interactions as our probe to estimate both the intensity B and the direction θ of the magnetic field when the probe reaches its steady state. We numerically calculate the quantum Fisher information (QFI) to characterize the estimation precision. On the one hand, for estimating B, we find that the coupling between spins in the probe plays an important role in the precision, and the largest value of the QFI can be achieved when θ = π/2 together with an optimal coupling. Moreover, for any direction, the precision scaling can be better than the Heisenberg-limit (HL) with a proper coupling. On the other hand, for estimating θ, we find that our probe can perform a high precision detection for θ ~ π/2, with the QFI much larger than that for any other directions, especially when the coupling is tuned to the optimal value. And we find that the precision scaling for θ ~ π/2 can be better than the HL, but for other directions, the precision scaling is only limited to the standard quantum limit (SQL). Due to the computational complexity we restrict the number of spins in the probe to 60.

  18. Interplay of spin-orbit coupling and superconducting correlations in germanium telluride thin films

    Energy Technology Data Exchange (ETDEWEB)

    Narayan, Vijay; Nguyen, Thuy-Anh; Mansell, Rhodri; Ritchie, David [Cavendish Laboratory, Department of Physics, University of Cambridge, J. J. Thomson Avenue, Cambridge, CB3 0HE (United Kingdom); Mussler, Gregor [Peter Gruenberg Institute (PGI-9), Forschungszentrum Juelich, 52425, Juelich (Germany)

    2016-03-15

    There is much current interest in combining superconductivity and spin-orbit coupling in order to induce the topological superconductor phase and associated Majorana-like quasiparticles which hold great promise towards fault-tolerant quantum computing. Experimentally these effects have been combined by the proximity-coupling of super-conducting leads and high spin-orbit materials such as InSb and InAs, or by controlled Cu-doping of topological insu-lators such as Bi{sub 2}Se{sub 3}. However, for practical purposes, a single-phase material which intrinsically displays both these effects is highly desirable. Here we demonstrate coexisting superconducting correlations and spin-orbit coupling in molecular-beam-epitaxy-grown thin films of GeTe. The former is evidenced by a precipitous low-temperature drop in the electrical resistivity which is quelled by a magnetic field, and the latter manifests as a weak antilocalisation (WAL) cusp in the magnetotransport. Our studies reveal several other intriguing features such as the presence of two-dimensional rather than bulk transport channels below 2 K, possible signatures of topological superconductivity, and unexpected hysteresis in the magnetotransport. Our work demonstrates GeTe to be a potential host of topological SC and Majorana-like excitations, and to be a versatile platform to develop quantum information device architectures. (copyright 2016 The Authors. Phys. Status Solidi RRL published by WILEY-VCH Verlag GmbH and Co. KGaA, Weinheim)

  19. Magnetic field sensing subject to correlated noise with a ring spin chain

    Science.gov (United States)

    Guo, Li-Sha; Xu, Bao-Ming; Zou, Jian; Shao, Bin

    2016-01-01

    In this paper, we focus on the magnetic field sensing subject to a correlated noise. We use a ring spin chain with only the nearest neighbor interactions as our probe to estimate both the intensity B and the direction θ of the magnetic field when the probe reaches its steady state. We numerically calculate the quantum Fisher information (QFI) to characterize the estimation precision. On the one hand, for estimating B, we find that the coupling between spins in the probe plays an important role in the precision, and the largest value of the QFI can be achieved when θ = π/2 together with an optimal coupling. Moreover, for any direction, the precision scaling can be better than the Heisenberg-limit (HL) with a proper coupling. On the other hand, for estimating θ, we find that our probe can perform a high precision detection for θ ~ π/2, with the QFI much larger than that for any other directions, especially when the coupling is tuned to the optimal value. And we find that the precision scaling for θ ~ π/2 can be better than the HL, but for other directions, the precision scaling is only limited to the standard quantum limit (SQL). Due to the computational complexity we restrict the number of spins in the probe to 60. PMID:27623048

  20. The effects of gap parameter and spin polarization on electronic Hartree and correlation energies of doped graphene nanoribbon

    Science.gov (United States)

    Rezania, Hamed; Abdi, Ameneh

    2017-04-01

    We study the behaviors of both Hartree and correlation energies of undoped gapped armchair graphene nanoribbon using random phase approximation in the context of Hubbard model Hamiltonian. Specially, the effects of spin polarization and gap parameter on electron density dependence of Hartree and correlation energies of armchair graphene nanoribbon has been addressed. Our results show the variation of gap parameter leads to considerable effect on correlation and Hartree energy behavior of spin unpolarized gapped graphene in the middle electron density region. However local Hubbard interaction parameter affects the behaviors of Hartree and correlation energy on the whole range of electron density in zero magnetization case. We also show that a considerable reduction has been observed for density dependence of Hartree and correlation energies of spin polarized gapped graphene nanoribbon.

  1. Sub-Shot-Noise Magnetometry with a Correlated Spin-Relaxation Dominated Alkali-Metal Vapor

    OpenAIRE

    Kominis, I. K.

    2007-01-01

    Spin noise sets fundamental limits to the precision of measurements using spin-polarized atomic vapors, such as performed with sensitive atomic magnetometers. Spin squeezing offers the possibility to extend the measurement precision beyond the standard quantum limit of uncorrelated atoms. Contrary to the current understanding, we show that even in the presence of spin relaxation, spin squeezing can lead to a significant reduction of spin noise, and hence an increase in magnetometric sensitivi...

  2. Nanoparticles of antiferromagnetic materials

    DEFF Research Database (Denmark)

    Madsen, Daniel Esmarch

    2008-01-01

    I denne Ph.D. afhandling studeres forskellige egenskaber ved antiferromagnetiske nanopartikler. I en ideel antiferromagnet er spinnene orienteret således at der ikke er et resulterende magnetisk moment. I nanopartikler af antiferromagnetiske materialer er denne kompensation på grund af forskellig...

  3. Macroscopic Quantum Coherence in Antiferromagnetic Molecular Magnets

    Institute of Scientific and Technical Information of China (English)

    HU Hui; LO Rong; ZHU Jia-Lin; XIONG Jia-Jiong

    2001-01-01

    The macroscopic quantum coherence in a biaxial antiferromagnetic molecular magnet in the presence of magnetic field acting parallel to its hard anisotropy axis is studied within the two-sublattice model. On the basis of instanton technique in the spin-coherent-state path-integral representation, both the rigorous Wentzel-Kramers-Brillouin exponent and pre-exponential factor for the ground-state tunnel splitting are obtained. We find that the quantum fluctuations around the classical paths can not only induce a new quantum phase previously reported by Chiolero and Loss (Phys. Rev. Lett. 80 (1998) 169), but also have great influence on the intensity of the ground-state tunnel splitting. Those features clearly have no analogue in the ferromagnetic molecular magnets. We suggest that they may be the universal behaviors in all antiferromagnetic molecular magnets. The analytical results are complemented by exact diagonalization calculation.

  4. Macroscopic Quantum Coherence in Antiferromagnetic Molecular Magnets

    Institute of Scientific and Technical Information of China (English)

    HUHui; LURong; 等

    2001-01-01

    The macroscopic quantum coherence in a biaxial antiferromagnetic molecular magnet in the presence of magnetic field acting parallel to its hard anisotropy axis is studied within the two-sublattice model.On the basis of instanton technique in the spin-coherent-state path-integral representation,both the rigorous Wentzel-Kramers-Brillouin exponent and pre-exponential factor for the ground-state tunnel splitting are obtained.We find that the quantum fluctuations around the classical paths can not only induce a new quantum phase previously reported by Chiolero and Loss (Phys.Rev.Lett.80(1998)169),but also have great influence on the intensity of the ground-state tunnel splitting.Those features clearly have no analogue in the ferromagnetic molecular magnets.We suggest that they may be the universal behaviors in all antiferromagnetic molecular magnets.The analytical results are complemented by exact diagonalization calculation.

  5. Local spin relaxation within the random Heisenberg chain.

    Science.gov (United States)

    Herbrych, J; Kokalj, J; Prelovšek, P

    2013-10-04

    Finite-temperature local dynamical spin correlations S(nn)(ω) are studied numerically within the random spin-1/2 antiferromagnetic Heisenberg chain. The aim is to explain measured NMR spin-lattice relaxation times in BaCu(2)(Si(0.5)Ge(0.5))(2)O(7), which is the realization of a random spin chain. In agreement with experiments we find that the distribution of relaxation times within the model shows a very large span similar to the stretched-exponential form. The distribution is strongly reduced with increasing T, but stays finite also in the high-T limit. Anomalous dynamical correlations can be associated with the random singlet concept but not directly with static quantities. Our results also reveal the crucial role of the spin anisotropy (interaction), since the behavior is in contrast with the ones for the XX model, where we do not find any significant T dependence of the distribution.

  6. Frustrated spin correlations in diluted spin ice Ho{sub 2-x}La{sub x}Ti{sub 2}O{sub 7}

    Energy Technology Data Exchange (ETDEWEB)

    Ehlers, G; Mamontov, E; Zamponi, M [Spallation Neutron Source, Oak Ridge National Laboratory, Building 8600, Oak Ridge, TN 37831-6475 (United States); Faraone, A; Qiu, Y [Department of Materials Science and Engineering, University of Maryland, College Park, MD 20742-2115 (United States); Cornelius, A L [Physics Department, University of Nevada Las Vegas, Las Vegas, NV 89154-4002 (United States); Booth, C H [Chemical Sciences Division, Lawrence Berkeley National Laboratory, Berkeley, CA 94720 (United States); Kam, K C; Toquin, R Le; Cheetham, A K [Materials Research Laboratory, University of California, Santa Barbara, CA 93106 (United States); Gardner, J S [NIST Center for Neutron Research, NIST, Gaithersburg, MD 20899-6102 (United States)], E-mail: ehlersg@ornl.gov

    2008-06-11

    We have studied the evolution of the structural properties as well as the static and dynamic spin correlations of spin ice Ho{sub 2}Ti{sub 2}O{sub 7}, where Ho was partially replaced by non-magnetic La. The crystal structure of diluted samples Ho{sub 2-x}La{sub x}Ti{sub 2}O{sub 7} was characterized by x-ray and neutron diffraction and by Ho L{sub III}-edge and Ti K-edge extended x-ray absorption fine structure (EXAFS) measurements. It is found that the pyrochlore structure remains intact until about x = 0.3, but a systematic increase in local disorder with increasing La concentration is observed in the EXAFS data, especially from the Ti K edge. Quasi-elastic neutron scattering and ac susceptibility measurements show that, in x{<=}0.4 samples at temperatures above macroscopic freezing, the spin-spin correlations are short ranged and dynamic in nature. The main difference with pure spin ice in the dynamics is the appearance of a second, faster, relaxation process.

  7. Overfrustrated and underfrustrated spin glasses in d =3 and 2: Evolution of phase diagrams and chaos including spin-glass order in d =2

    Science.gov (United States)

    Ilker, Efe; Berker, A. Nihat

    2014-04-01

    In spin-glass systems, frustration can be adjusted continuously and considerably, without changing the antiferromagnetic bond probability p, by using locally correlated quenched randomness, as we demonstrate here on hypercubic lattices and hierarchical lattices. Such overfrustrated and underfrustrated Ising systems on hierarchical lattices in d =3 and 2 are studied. With the removal of just 51% of frustration, a spin-glass phase occurs in d =2. With the addition of just 33% frustration, the spin-glass phase disappears in d =3. Sequences of 18 different phase diagrams for different levels of frustration are calculated in both dimensions. In general, frustration lowers the spin-glass ordering temperature. At low temperatures, increased frustration favors the spin-glass phase (before it disappears) over the ferromagnetic phase and symmetrically the antiferromagnetic phase. When any amount, including infinitesimal, frustration is introduced, the chaotic rescaling of local interactions occurs in the spin-glass phase. Chaos increases with increasing frustration, as can be seen from the increased positive value of the calculated Lyapunov exponent λ, starting from λ =0 when frustration is absent. The calculated runaway exponent yR of the renormalization-group flows decreases with increasing frustration to yR=0 when the spin-glass phase disappears. From our calculations of entropy and specific-heat curves in d =3, it is shown that frustration lowers in temperature the onset of both long- and short-range order in spin-glass phases, but is more effective on the former. From calculations of the entropy as a function of antiferromagnetic bond concentration p, it is shown that the ground-state and low-temperature entropy already mostly sets in within the ferromagnetic and antiferromagnetic phases, before the spin-glass phase is reached.

  8. Overfrustrated and underfrustrated spin glasses in d=3 and 2: evolution of phase diagrams and chaos including spin-glass order in d=2.

    Science.gov (United States)

    Ilker, Efe; Berker, A Nihat

    2014-04-01

    In spin-glass systems, frustration can be adjusted continuously and considerably, without changing the antiferromagnetic bond probability p, by using locally correlated quenched randomness, as we demonstrate here on hypercubic lattices and hierarchical lattices. Such overfrustrated and underfrustrated Ising systems on hierarchical lattices in d=3 and 2 are studied. With the removal of just 51% of frustration, a spin-glass phase occurs in d=2. With the addition of just 33% frustration, the spin-glass phase disappears in d=3. Sequences of 18 different phase diagrams for different levels of frustration are calculated in both dimensions. In general, frustration lowers the spin-glass ordering temperature. At low temperatures, increased frustration favors the spin-glass phase (before it disappears) over the ferromagnetic phase and symmetrically the antiferromagnetic phase. When any amount, including infinitesimal, frustration is introduced, the chaotic rescaling of local interactions occurs in the spin-glass phase. Chaos increases with increasing frustration, as can be seen from the increased positive value of the calculated Lyapunov exponent λ, starting from λ=0 when frustration is absent. The calculated runaway exponent yR of the renormalization-group flows decreases with increasing frustration to yR=0 when the spin-glass phase disappears. From our calculations of entropy and specific-heat curves in d=3, it is shown that frustration lowers in temperature the onset of both long- and short-range order in spin-glass phases, but is more effective on the former. From calculations of the entropy as a function of antiferromagnetic bond concentration p, it is shown that the ground-state and low-temperature entropy already mostly sets in within the ferromagnetic and antiferromagnetic phases, before the spin-glass phase is reached.

  9. Symmetry Reduction in the Quantum Kagome Antiferromagnet Herbertsmithite

    Science.gov (United States)

    Zorko, A.; Herak, M.; Gomilšek, M.; van Tol, J.; Velázquez, M.; Khuntia, P.; Bert, F.; Mendels, P.

    2017-01-01

    Employing complementary torque magnetometry and electron spin resonance on single crystals of herbertsmithite, the closest realization to date of a quantum kagome antiferromagnet featuring a spin-liquid ground state, we provide novel insight into different contributions to its magnetism. At low temperatures, two distinct types of defects with different magnetic couplings to the kagome spins are found. Surprisingly, their magnetic response contradicts the threefold symmetry of the ideal kagome lattice, suggesting the presence of a global structural distortion that may be related to the establishment of the spin-liquid ground state.

  10. Observation of Antiferromagnetic Resonance in an Organic Superconductor

    DEFF Research Database (Denmark)

    Torrance, J. B.; Pedersen, H. J.; Bechgaard, K.

    1982-01-01

    Anomalous microwave absorption has been observed in the organic superconductor TMTSF2AsF6 (TMTSF: tetramethyltetraselenafulvalene) below its metal-nonmetal transition near 12 K. This absorption is unambiguously identified as antiferromagnetic resonance by the excellent agreement between a spin...

  11. Non-Markovian spin-resolved counting statistics and an anomalous relation between autocorrelations and cross correlations in a three-terminal quantum dot

    Science.gov (United States)

    Luo, JunYan; Yan, Yiying; Huang, Yixiao; Yu, Li; He, Xiao-Ling; Jiao, HuJun

    2017-01-01

    We investigate the noise correlations of spin and charge currents through an electron spin resonance (ESR)-pumped quantum dot, which is tunnel coupled to three electrodes maintained at an equivalent chemical potential. A recursive scheme is employed with inclusion of the spin degrees of freedom to account for the spin-resolved counting statistics in the presence of non-Markovian effects due to coupling with a dissipative heat bath. For symmetric spin-up and spin-down tunneling rates, an ESR-induced spin flip mechanism generates a pure spin current without an accompanying net charge current. The stochastic tunneling of spin carriers, however, produces universal shot noises of both charge and spin currents, revealing the effective charge and spin units of quasiparticles in transport. In the case of very asymmetric tunneling rates for opposite spins, an anomalous relationship between noise autocorrelations and cross correlations is revealed, where super-Poissonian autocorrelation is observed in spite of a negative cross correlation. Remarkably, with strong dissipation strength, non-Markovian memory effects give rise to a positive cross correlation of the charge current in the absence of a super-Poissonian autocorrelation. These unique noise features may offer essential methods for exploiting internal spin dynamics and various quasiparticle tunneling processes in mesoscopic transport.

  12. Nematic antiferromagnetic states in bulk FeSe

    Science.gov (United States)

    Liu, Kai; Lu, Zhong-Yi; Xiang, Tao

    2016-05-01

    The existence of nematic order, which breaks the lattice rotational symmetry with nonequivalent a and b axes in iron-based superconductors, is a well-established experimental fact. An antiferromagnetic (AFM) transition is accompanying this order, observed in nearly all parent compounds, except bulk FeSe. The absence of the AFM order in FeSe casts doubt on the magnetic mechanism of iron-based superconductivity, since the nematic order is believed to be driven by the same interaction that is responsible for the superconducting pairing in these materials. Here we show, through systematic first-principles electronic structure calculations, that the ground state of FeSe is in fact strongly AFM correlated but without developing a magnetic long-range order. Actually, there are a series of staggered n -mer AFM states with corresponding energies below that of the single stripe AFM state, which is the ground state for the parent compounds of most iron-based superconductors. Here, the staggered n -mer (n any integer >1 ) means a set of n adjacent parallel spins on a line along the b axis with antiparallel spins between n -mers along both a and b axes. Moreover, different n -mers can antiparallelly mix with each other to coexist. Among all the states, we find that the lowest energy states formed by the staggered dimer, staggered trimer, and their random antiparallel aligned spin states along the b axis are quasidegenerate. The thermal average of these states does not show any magnetic long-range order, but it does possess a hidden one-dimensional AFM order along the a axis, which can be detected by elastic neutron scattering measurements. Our finding gives a natural account for the absence of long-range magnetic order and suggests that the nematicity is driven predominantly by spin fluctuations even in bulk FeSe, providing a unified description on the phase diagram of iron-based superconductors.

  13. Characterization of the Dilute Ising Antiferromagnet

    Energy Technology Data Exchange (ETDEWEB)

    Wiener, T.

    2000-09-12

    A spin glass is a magnetic ground state in which ferromagnetic and antiferromagnetic exchange interactions compete, thereby creating frustration and a multidegenerate state with no long range order. An Ising system is a system where the spins are constrained to lie parallel or antiparallel to a primary axis. There has been much theoretical interest in the past ten years in the effects of applying a magnetic field transverse to the primary axis in an Ising spin glass at low temperatures and thus study phase transitions at the T=0 limit. The focus of this study is to search for and characterize a new Ising spin glass system. This is accomplished by site diluting yttrium for terbium in the crystalline material TbNi{sub 2}Ge{sub 2}. The first part of this work gives a brief overview of the physics of rare earth magnetism and an overview of experimental characteristics of spin glasses. This is followed by the methodology used to manufacture the large single crystals used in this study, as well as the measurement techniques used. Next, a summary of the results of magnetic measurements on across the dilution series from pure terbium to pure yttrium is presented. This is followed by detailed measurements on particular dilutions which demonstrate spin glass behavior. Pure TbNi{sub 2}Ge{sub 2} is an Ising antiferromagnet with a several distinct metamagnetic states below 17 K. As the terbium is alloyed with yttrium, these magnetic states are weakened in a consistent manner, as is seen in measurements of the transition temperatures and analysis of Curie-Weiss behavior at high temperature. At low concentrations of terbium, below 35%, long range order is no longer present and a spin-glass-like state emerges. This state is studied through various measurements, dc and ac susceptibility, resistivity, and specific heat. This magnetic behavior was then compared to that of other well characterized spin glasses. It is concluded that there is a region of concentration s for which a spin

  14. Characterization of the Dilute Ising Antiferromagnet

    Energy Technology Data Exchange (ETDEWEB)

    Wiener, Timothy [Iowa State Univ., Ames, IA (United States)

    2000-09-12

    A spin glass is a magnetic ground state in which ferromagnetic and antiferromagnetic exchange interactions compete, thereby creating frustration and a multidegenerate state with no long range order. An Ising system is a system where the spins are constrained to lie parallel or antiparallel to a primary axis. There has been much theoretical interest in the past ten years in the effects of applying a magnetic field transverse to the primary axis in an Ising spin glass at low temperatures and thus study phase transitions at the T=0 limit. The focus of this study is to search for and characterize a new Ising spin glass system. This is accomplished by site diluting yttrium for terbium in the crystalline material TbNi2Ge2. The first part of this work gives a brief overview of the physics of rare earth magnetism and an overview of experimental characteristics of spin glasses. This is followed by the methodology used to manufacture the large single crystals used in this study, as well as the measurement techniques used. Next, a summary of the results of magnetic measurements on across the dilution series from pure terbium to pure yttrium is presented. This is followed by detailed measurements on particular dilutions which demonstrate spin glass behavior. Pure TbNi2Ge2 is an Ising antiferromagnet with a several distinct metamagnetic states below 17 K. As the terbium is alloyed with yttrium, these magnetic states are weakened in a consistent manner, as is seen in measurements of the transition temperatures and analysis of Curie-Weiss behavior at high temperature. At low concentrations of terbium, below 35%, long range order is no longer present and a spin-glass-like state emerges. This state is studied through various measurements, dc and ac susceptibility, resistivity, and specific heat. This magnetic behavior was then compared to that of other well characterized spin glasses. It is concluded that there is a region of

  15. Holes in Heisenberg antiferromagnets

    Science.gov (United States)

    Chen, Yang

    1990-05-01

    In this Brief Report we show that a recent model proposed by Shankar [Phys. Rev. Lett. 63, 203 (1989)], describing the motion of holes in quantum antiferromagnets is equivalent to the Schwinger model [Phys. Rev. 128, 2425 (1962)] in 1+1 dimensions. Some exact results are deduced. In addition to the superconducting long-range order found by Shankar, it is shown that there is a 2pF hole density wave existing with the superconducting pairing instability.

  16. Switching of antiferromagnetic chains with magnetic pulses

    Science.gov (United States)

    Tao, Kun; Polyakov, Oleg P.; Stepanyuk, Valeri S.

    2016-04-01

    Recent experimental studies have demonstrated the possibility of information storage in short antiferromagnetic chains on an insulator substrate [S. Loth et al., Science 335, 196 (2012), 10.1126/science.1214131]. Here, using the density functional theory and atomistic spin dynamics simulations, we show that a local magnetic control of such chains with a magnetic tip and magnetic pulses can be used for fast switching of their magnetization. Furthermore, by changing the position of the tip one can engineer the magnetization dynamics of the chains.

  17. Analysing powers and spin correlations in deuteron-proton charge exchange at 726 MeV

    CERN Document Server

    Dymov, S; Bagdasarian, Z; Barsov, S; Carbonell, J; Chiladze, D; Engels, R; Gebel, R; Grigoryev, K; Hartmann, M; Kacharava, A; Khoukaz, A; Komarov, V; Kulessa, P; Kulikov, A; Kurbatov, V; Lomidze, N; Lorentz, B; Macharashvili, G; Mchedlishvili, D; Merzliakov, S; Mielke, M; Mikirtychyants, M; Mikirtychyants, S; Nioradze, M; Ohm, H; Prasuhn, D; Rathmann, F; Serdyuk, V; Seyfarth, H; Shmakova, V; Ströher, H; Tabidze, M; Trusov, S; Tsirkov, D; Uzikov, Yu; Valdau, Yu; Weidemann, C; Wilkin, C

    2015-01-01

    The charge exchange of vector polarised deuterons on a polarised hydrogen target has been studied in a high statistics experiment at the COSY-ANKE facility at a deuteron beam energy of Td = 726 MeV. By selecting two fast protons at low relative energy E_{pp}, the measured analysing powers and spin correlations are sensitive to interference terms between specific neutron-proton charge-exchange amplitudes at a neutron kinetic energy of Tn ~ 1/2 Td =363 MeV. An impulse approximation calculation, which takes into account corrections due to the angular distribution in the diproton, describes reasonably the dependence of the data on both E_{pp} and the momentum transfer. This lends broad support to the current neutron-proton partial-wave solution that was used in the estimation.

  18. Analysing powers and spin correlations in deuteron–proton charge exchange at 726 MeV

    Directory of Open Access Journals (Sweden)

    S. Dymov

    2015-05-01

    Full Text Available The charge exchange of vector polarised deuterons on a polarised hydrogen target has been studied in a high statistics experiment at the COSY-ANKE facility at a deuteron beam energy of Td=726 MeV. By selecting two fast protons at low relative energy Epp, the measured analysing powers and spin correlations are sensitive to interference terms between specific neutron–proton charge-exchange amplitudes at a neutron kinetic energy of Tn≈12Td=363 MeV. An impulse approximation calculation, which takes into account corrections due to the angular distribution in the diproton, describes reasonably the dependence of the data on both Epp and the momentum transfer. This lends broad support to the current neutron–proton partial wave solution that was used in the estimation.

  19. Volume localized spin echo correlation spectroscopy with suppression of 'diagonal' peaks.

    Science.gov (United States)

    Banerjee, Abhishek; Chandrakumar, N

    2014-02-01

    Two dimensional homonuclear (1)H correlation spectroscopy is of considerable interest for volume localized spectral studies, both in vivo and in vitro, of biological as well as material objects. The information principally sought from correlation spectra resides in the cross-peaks, which are often masked however by the presence of diagonal peaks in COSY, or 'pseudo-diagonal' peaks at F1=0 in SECSY. It has therefore been a concern to suppress these diagonal or 'pseudo-diagonal' peaks, in order to ensure that cross-peak information is fully discernible. We present here a report of our work on volume localized DIagonal Suppressed Spin Echo Correlation specTroscopy (LDISSECT) and demonstrate its performance in comparison to the standard volume localized SECSY experiment, employing brain metabolite phantoms in a gel. The sequence works in the inhomogeneous, multi-component environment by exploiting the short acquisition time to suppress undesired information by employing an additional rf pulse. A brief description of the pulse sequence, its theory, and simulations are also included, besides experimental benchmarking on two brain metabolite phantoms in gel phase.

  20. Quantifying the importance of orbital over spin correlations in delta-Pu within density-functional theory

    Energy Technology Data Exchange (ETDEWEB)

    Soderlind, P; Wolfer, W

    2007-07-27

    Spin and orbital and electron correlations are known to be important when treating the high-temperature {delta} phase of plutonium within the framework of density-functional theory (DFT). One of the more successful attempts to model {delta}-Pu within this approach has included condensed-matter generalizations of Hund's three rules for atoms, i.e., spin polarization, orbital polarization, and spin-orbit coupling. Here they perform a quantitative analysis of these interactions relative rank for the bonding and electronic structure in {delta}-Pu within the DFT model. The result is somewhat surprising in that spin-orbit coupling and orbital polarization are far more important than spin polarization for a realistic description of {delta}-Pu. They show that these orbital correlations on their own, without any formation of magnetic spin moments, can account for the low atomic density of the {delta} phase with a reasonable equation-of-state. In addition, this unambiguously non-magnetic (NM) treatment produces a one-electron spectra with resonances close to the Fermi level consistent with experimental valence band photoemission spectra.

  1. Anisotropy of electron and hole g tensors of quantum dots: An intuitive picture based on spin-correlated orbital currents

    Science.gov (United States)

    van Bree, J.; Silov, A. Yu.; van Maasakkers, M. L.; Pryor, C. E.; Flatté, M. E.; Koenraad, P. M.

    2016-01-01

    Using single spins in semiconductor quantum dots as qubits requires full control over the spin state. As the g tensor provides the coupling in a Hamiltonian between a spin and an external magnetic field, a deeper understanding of the g tensor underlies magnetic-field control of the spin. The g tensor is affected by the presence of spin-correlated orbital currents, of which the spatial structure has been recently clarified. Here we extend that framework to investigate the influence of the shape of quantum dots on the anisotropy of the electron g tensor. We find that the spin-correlated orbital currents form a simple current loop perpendicular to the magnetic moment's orientation. The current loop is therefore directly sensitive to the shape of the nanostructure: for cylindrical quantum dots, the electron g -tensor anisotropy is mainly governed by the aspect ratio of the dots. Through a systematic experimental study of the size dependence of the separate electron and hole g tensors of InAs/InP quantum dots, we have validated this picture. Moreover, we find that through size engineering it is possible to independently change the sign of the in-plane and growth direction electron g factors. The hole g tensor is found to be strongly anisotropic and very sensitive to the radius and elongation. The comparable importance of itinerant and localized currents to the hole g tensor complicates the analysis relative to the electron g tensor.

  2. Effective mapping of spin-1 chains onto integrable fermionic models. A study of string and Neel correlation functions

    Energy Technology Data Exchange (ETDEWEB)

    Boschi, C Degli Esposti [CNR, Unita CNISM di Bologna, viale Berti-Pichat, 6/2, I-40127, Bologna (Italy); Di Dio, M; Morandi, G [Dipartimento di Fisica dell' Universita di Bologna, viale Berti-Pichat, 6/2, I-40127, Bologna (Italy); Roncaglia, M [Max-Planck-Institut fuer Quantenoptik, Hans-Kopfermann-Str. 1, D-85748, Garching (Germany)

    2009-02-06

    We derive the dominant contribution to the large-distance decay laws of correlation functions towards their asymptotic limits for a spin chain model that exhibits both Haldane and Neel phases in its ground-state phase diagram. The analytic results are obtained by means of an approximate mapping between a spin-1 anisotropic Hamiltonian onto a fermionic model of noninteracting Bogoliubov quasiparticles related in turn (via Jordan-Wigner transformation) to the XY spin-1/2 chain in a transverse field. This approach allows us to express the spin-1 string operators in terms of fermionic operators so that the dominant contribution to the string correlators at large distances can be computed using the technique of Toeplitz determinants. As expected, we find long-range string order both in the longitudinal and in the transverse channel in the Haldane phase, while in the Neel phase only the longitudinal order survives. In this way, the long-range string order can be explicitly related to the components of the magnetization of the XY model. Moreover, apart from the critical line, where the decay is algebraic, we find that in the gapped phases the decay is governed by an exponential tail multiplied by power-law factors. As regards the usual two points correlation functions, we show that the longitudinal one behaves in a 'dual' fashion with respect to the transverse string correlator, namely both the asymptotic values and the decay laws exchange when the transition line is crossed. For the transverse spin-spin correlator, we always find a finite characteristic length which is an unexpected feature at the critical point. The results of this analysis prove some conjectures put forward in the past. We also comment briefly on the entanglement features of the original system versus those of the effective model. The goodness of the approximation and the analytical predictions are checked versus density-matrix renormalization group calculations.

  3. Antiferromagnetic hedgehogs with superconducting cores

    Energy Technology Data Exchange (ETDEWEB)

    Goldbart, P.M.; Sheehy, D.E. [Department of Physics and Materials Research Laboratory, University of Illinois at Urbana-Champaign, Urbana, Illinois 61801 (United States)

    1998-09-01

    Excitations of the antiferromagnetic state that resemble antiferromagnetic hedgehogs at large distances but are predominantly superconducting inside a core region are discussed within the context of Zhang{close_quote}s SO(5)-symmetry-based approach to the physics of high-temperature superconducting materials. Nonsingular, in contrast with their hedgehog cousins in pure antiferromagnetism, these texture excitations are what hedgehogs become when the antiferromagnetic order parameter is permitted to {open_quotes}escape{close_quotes} into superconducting directions. The structure of such excitations is determined in a simple setting, and a number of their experimental implications are examined. {copyright} {ital 1998} {ital The American Physical Society}

  4. Relativistic Néel-Order Fields Induced by Electrical Current in Antiferromagnets

    KAUST Repository

    Železný, J.

    2014-10-06

    We predict that a lateral electrical current in antiferromagnets can induce nonequilibrium Néel-order fields, i.e., fields whose sign alternates between the spin sublattices, which can trigger ultrafast spin-axis reorientation. Based on microscopic transport theory calculations we identify staggered current-induced fields analogous to the intraband and to the intrinsic interband spin-orbit fields previously reported in ferromagnets with a broken inversion-symmetry crystal. To illustrate their rich physics and utility, we consider bulk Mn2Au with the two spin sublattices forming inversion partners, and a 2D square-lattice antiferromagnet with broken structural inversion symmetry modeled by a Rashba spin-orbit coupling. We propose an antiferromagnetic memory device with electrical writing and reading.

  5. Antiferromagnetic proximity effect in epitaxial CoO/NiO/MgO(001) systems.

    Science.gov (United States)

    Li, Q; Liang, J H; Luo, Y M; Ding, Z; Gu, T; Hu, Z; Hua, C Y; Lin, H-J; Pi, T W; Kang, S P; Won, C; Wu, Y Z

    2016-03-02

    Magnetic proximity effect between two magnetic layers is an important focus of research for discovering new physical properties of magnetic systems. Antiferromagnets (AFMs) are fundamental systems with magnetic ordering and promising candidate materials in the emerging field of antiferromagnetic spintronics. However, the magnetic proximity effect between antiferromagnetic bilayers is rarely studied because detecting the spin orientation of AFMs is challenging. Using X-ray linear dichroism and magneto-optical Kerr effect measurements, we investigated antiferromagnetic proximity effects in epitaxial CoO/NiO/MgO(001) systems. We found the antiferromagnetic spin of the NiO underwent a spin reorientation transition from in-plane to out-of-plane with increasing NiO thickness, with the existence of vertical exchange spring spin alignment in thick NiO. More interestingly, the Néel temperature of the CoO layer was greatly enhanced by the adjacent NiO layer, with the extent of the enhancement closely dependent on the spin orientation of NiO layer. This phenomenon was attributed to different exchange coupling strengths at the AFM/AFM interface depending on the relative spin directions. Our results indicate a new route for modifying the spin configuration and ordering temperature of AFMs through the magnetic proximity effect near room temperature, which should further benefit the design of AFM spintronic devices.

  6. Oxygen-molecule spin-nanotubes constructed by physisorption into a nanoporous medium

    Science.gov (United States)

    Mito, Masaki; Shinto, Noritoshi; Komorida, Yuki; Tajiri, Takayuki; Deguchi, Hiroyuki; Takagi, Seishi; Kohiki, Shigemi

    2008-08-01

    We succeeded in controlling gas-liquid-solid transitions and in constructing “spin-nanotubes (SNTs)” based on antiferromagnetic correlations by physisorbing oxygen molecules (O2) into the nanosize pores of a mesoporous medium MCM-41 while also manipulating the adsorption quantity. The phase diagram of O2 physisorbed into MCM-41 presents many common characteristics with that of O2 layers physisorbed on graphite substrates. In the present case, experimental verification of the antiferromagnetic square lattice in the liquid phase of the monolayer proved the formation of O2 SNTs. The present O2 SNT is an experimental example of the successful construction of SNT.

  7. Spin-orbit interaction in quantum dots and quantum wires of correlated electrons - a way to spintronics?

    Energy Technology Data Exchange (ETDEWEB)

    Birkholz, Jens Eiko

    2008-10-06

    We study the influence of the spin-orbit interaction on the electronic transport through quantum dots and quantum wires of correlated electrons. Starting with a one-dimensional infinite continuum model without Coulomb interaction, we analyze the interplay of the spin-orbit interaction, an external magnetic field, and an external potential leading to currents with significant spin-polarization in appropriate parameter regimes. Since lattice models are known to often be superior to continuum models in describing the experimental situation of low-dimensional mesoscopic systems, we construct a lattice model which exhibits the same low-energy physics in terms of energy dispersion and spin expectation values. Confining the lattice to finite length and connecting it to two semi-infinite noninteracting Fermi liquid leads, we calculate the zero temperature linear conductance using the Landauer-Bttiker formalism and show that spin-polarization effects also evolve for the lattice model by adding an adequate potential structure and can be controlled by tuning the overall chemical potential of the system (quantum wire and leads). Next, we allow for a finite Coulomb interaction and use the functional renormalization group (fRG) method to capture correlation effects induced by the Coulomb interaction. The interacting system is thereby transformed into a noninteracting system with renormalized system parameters. For short wires ({proportional_to}100 lattice sites), we show that the energy regime in which spin polarization is found is strongly affected by the Coulomb interaction. For long wires (>1000 lattice sites), we find the power-law suppression of the total linear conductance on low energy scales typical for inhomogeneous Luttinger liquids while the degree of spin polarization stays constant. Considering quantum dots which consist of two lattice sites, we observe the well-known Kondo effect and analyze, how the Kondo temperature is affected by the spin-orbit interaction

  8. Antiferromagnetic order of strongly interacting fermions in a trap: real-space dynamical mean-field analysis

    Energy Technology Data Exchange (ETDEWEB)

    Snoek, M; Titvinidze, I; Toeke, C; Hofstetter, W [Institut fuer Theoretische Physik, Johann Wolfgang Goethe-Universitaet, 60438 Frankfurt/Main (Germany); Byczuk, K [Theoretical Physics III, Center for Electronic Correlations and Magnetism, Institute for Physics, University of Augsburg, 86135 Augsburg (Germany)], E-mail: snoek@itp.uni-frankfurt.de

    2008-09-15

    We apply dynamical mean-field theory to strongly interacting fermions in an inhomogeneous environment. With the help of this real-space dynamical mean-field theory (R-DMFT) we investigate antiferromagnetic states of repulsively interacting fermions with spin1/2 in a harmonic potential. Within R-DMFT, antiferromagnetic order is found to be stable in spatial regions with total particle density close to one, but persists also in parts of the system where the local density significantly deviates from half filling. In systems with spin imbalance, we find that antiferromagnetism is gradually suppressed and phase separation emerges beyond a critical value of the spin imbalance.

  9. Analyzing powers and spin correlations ANN and ALL for pp-->npπ+ at 650 and 800 MeV

    Science.gov (United States)

    Bhatia, T. S.; Boissevain, J. G. J.; Jarmer, J. J.; Silbar, R. R.; Simmons, J. E.; Glass, G.; Hiebert, J. C.; Kenefick, R. A.; Northcliffe, L. C.; Tippens, W. B.; Kloet, W. M.; Dubach, J.

    1983-11-01

    We report first measurements of the spin correlation parameters, ANN and ALL, for pp-->npπ+ above the Δ-production threshold. Our results for this dominant inelastic channel are in good agreement with a theoretical model that does not include any dibaryon resonances.

  10. Spin Correlations in the $\\Lambda \\Lambda$ and $\\Lambda \\Lambda¯$ Systems Generated in Relativistic Heavy-Ion Collisions

    CERN Document Server

    Lyuboshitz, V L

    2010-01-01

    Spin correlations for the and ¯ pairs, generated in relativistic heavy ion collisions, and related angular correlations at the joint registration of hadronic decays of two hyperons with non-conservation of space parity are analyzed. Within the conventional model of oneparticle sources, correlations vanish at enough large relative momenta. However, under these conditions, in the case of two non-identical particles ( ¯ ) a noticeable role is played by two-particle annihilation (two-quark, two-gluon) sources, which lead to the difference of the correlation tensor from zero. In particular, such a situation may arise when the system passes through the “mixed phase”.

  11. Antiferromagnetic phase diagram of the cuprate superconductors

    Science.gov (United States)

    Nunes, L. H. C. M.; Teixeira, A. W.; Marino, E. C.

    2017-02-01

    Taking the spin-fermion model as the starting point for describing the cuprate superconductors, we obtain an effective nonlinear sigma-field hamiltonian, which takes into account the effect of doping in the system. We obtain an expression for the spin-wave velocity as a function of the chemical potential. For appropriate values of the parameters we determine the antiferromagnetic phase diagram for the YBa2Cu3O6+x compound as a function of the dopant concentration in good agreement with the experimental data. Furthermore, our approach provides a unified description for the phase diagrams of the hole-doped and the electron doped compounds, which is consistent with the remarkable similarity between the phase diagrams of these compounds, since we have obtained the suppression of the antiferromagnetic phase as the modulus of the chemical potential increases. The aforementioned result then follows by considering positive values of the chemical potential related to the addition of holes to the system, while negative values correspond to the addition of electrons.

  12. Variable Spin-Down in the Soft Gamma Repeater SGR 1900+14 and Correlations with Burst Activity

    Science.gov (United States)

    Woods, Peter M.; Kouveliotou, Chryssa; VanParadijs, Jan; Finger, Mark H.; Thompson, Christopher; Duncan, Robert C.; Hurley, Kevin; Strohmayer, Tod; Swank, Jean; Murakami, Toshio

    1999-01-01

    We have analyzed Rossi X-ray Timing Explorer Proportional Counter Array observations of the pulsed emission from SGR 1900+ 14 during 1996 September, 1998 June-October, and early 1999. Using these measurements and results reported elsewhere, we construct a period history of this source for 2.5 yr. We find significant deviations from a steady spin-down trend during quiescence and the burst active interval. Burst and Transient Source Experiment observations of the burst emission are presented and correlations between the burst activity and spin-down rate of SGR 1900+14 are discussed. We find an 80 day interval during the summer of 1998 when the average spin-down rate is larger than the rate elsewhere by a factor approximately 2.3. This enhanced spin-down may be the result of a discontinuous spin-down event or "braking glitch" at the time of the giant flare on 1998 August 27. Furthermore, we find a large discrepancy between the pulsar period and average spin-down rate in X-rays as compared to radio observations for 1998 December and 1999 January.

  13. Ferrimagnetism in delta chain with anisotropic ferromagnetic and antiferromagnetic interactions

    Science.gov (United States)

    Dmitriev, D. V.; Krivnov, V. Ya

    2016-12-01

    We consider analytically and numerically an anisotropic spin-\\frac{1}{2} delta-chain (sawtooth chain) in which exchange interactions between apical and basal spins are ferromagnetic and those between basal spins are antiferromagnetic. In the limit of strong anisotropy of exchange interactions this model can be considered as the Ising delta chain with macroscopic degenerate ground state perturbed by transverse quantum fluctuations. These perturbations lift the ground state degeneracy and the model reduces to the basal XXZ spin chain in the magnetic field induced by static apical spins. We show that the ground state of such a model is ferrimagnetic. The excitations of the model are formed by ferrimagnetic domains separated by domain walls with a finite energy. At low temperatures the system is effectively divided into two independent subsystems, the apical subsystem described by the Ising spin-\\frac{1}{2} chain and the basal subsystem described by the XXZ chain with infinite zz interactions.

  14. Spin dynamics simulations of topological magnon insulators: From transverse current correlation functions to the family of magnon Hall effects

    Science.gov (United States)

    Mook, Alexander; Henk, Jürgen; Mertig, Ingrid

    2016-11-01

    We demonstrate theoretically that atomistic spin dynamics simulations of topological magnon insulators (TMIs) provide access to the magnon-mediated transport of both spin and heat. The TMIs, modeled by kagome ferromagnets with Dzyaloshinskii-Moriya interaction, exhibit nonzero transverse-current correlation functions from which conductivities are derived for the entire family of magnon Hall effects. Both longitudinal and transverse conductivities are studied in dependence on temperature and on an external magnetic field. A comparison between theoretical and experimental results for Cu(1,3-benzenedicarboxylate), a recently discovered TMI, is drawn.

  15. Electrical switching of an antiferromagnet.

    Science.gov (United States)

    Wadley, P; Howells, B; Železný, J; Andrews, C; Hills, V; Campion, R P; Novák, V; Olejník, K; Maccherozzi, F; Dhesi, S S; Martin, S Y; Wagner, T; Wunderlich, J; Freimuth, F; Mokrousov, Y; Kuneš, J; Chauhan, J S; Grzybowski, M J; Rushforth, A W; Edmonds, K W; Gallagher, B L; Jungwirth, T

    2016-02-05

    Antiferromagnets are hard to control by external magnetic fields because of the alternating directions of magnetic moments on individual atoms and the resulting zero net magnetization. However, relativistic quantum mechanics allows for generating current-induced internal fields whose sign alternates with the periodicity of the antiferromagnetic lattice. Using these fields, which couple strongly to the antiferromagnetic order, we demonstrate room-temperature electrical switching between stable configurations in antiferromagnetic CuMnAs thin-film devices by applied current with magnitudes of order 10(6) ampere per square centimeter. Electrical writing is combined in our solid-state memory with electrical readout and the stored magnetic state is insensitive to and produces no external magnetic field perturbations, which illustrates the unique merits of antiferromagnets for spintronics.

  16. Magnetic phase diagrams of classical triangular and kagome antiferromagnets

    Energy Technology Data Exchange (ETDEWEB)

    Gvozdikova, M V [Department of Physics, Kharkov National University, 61077 Kharkov (Ukraine); Melchy, P-E; Zhitomirsky, M E, E-mail: mike.zhitomirsky@cea.fr [Service de Physique Statistique, Magnetisme et Supraconductivite, UMR-E9001 CEA-INAC/UJF, 17 rue des Martyrs, 38054 Grenoble (France)

    2011-04-27

    We investigate the effect of geometrical frustration on the H-T phase diagrams of the classical Heisenberg antiferromagnets on triangular and kagome lattices. The phase diagrams for the two models are obtained from large-scale Monte Carlo simulations. For the kagome antiferromagnet, thermal fluctuations are unable to lift degeneracy completely and stabilize translationally disordered multipolar phases. We find a substantial difference in the temperature scales of the order by disorder effect related to different degeneracy of the low- and the high-field classical ground states in the kagome antiferromagnet. In the low-field regime, the Kosterlitz-Thouless transition into a spin-nematic phase is produced by unbinding of half-quantum vortices.

  17. Magnetic phase diagrams of classical triangular and kagome antiferromagnets.

    Science.gov (United States)

    Gvozdikova, M V; Melchy, P-E; Zhitomirsky, M E

    2011-04-27

    We investigate the effect of geometrical frustration on the H-T phase diagrams of the classical Heisenberg antiferromagnets on triangular and kagome lattices. The phase diagrams for the two models are obtained from large-scale Monte Carlo simulations. For the kagome antiferromagnet, thermal fluctuations are unable to lift degeneracy completely and stabilize translationally disordered multipolar phases. We find a substantial difference in the temperature scales of the order by disorder effect related to different degeneracy of the low- and the high-field classical ground states in the kagome antiferromagnet. In the low-field regime, the Kosterlitz-Thouless transition into a spin-nematic phase is produced by unbinding of half-quantum vortices.

  18. Revealing the properties of Mn2Au for antiferromagnetic spintronics.

    Science.gov (United States)

    Barthem, V M T S; Colin, C V; Mayaffre, H; Julien, M-H; Givord, D

    2013-01-01

    The continuous reduction in size of spintronic devices requires the development of structures, which are insensitive to parasitic external magnetic fields, while preserving the magnetoresistive signals of existing systems based on giant or tunnel magnetoresistance. This could be obtained in tunnel anisotropic magnetoresistance structures incorporating an antiferromagnetic, instead of a ferromagnetic, material. To turn this promising concept into real devices, new magnetic materials with large spin-orbit effects must be identified. Here we demonstrate that Mn2Au is not a Pauli paramagnet as hitherto believed but an antiferromagnet with Mn moments of ~4 μB. The particularly large strength of the exchange interactions leads to an extrapolated Néel temperature well above 1,000 K, so that ground-state magnetic properties are essentially preserved up to room temperature and above. Combined with the existence of a significant in-plane anisotropy, this makes Mn2Au the most promising material for antiferromagnetic spintronics identified so far.

  19. Spin-triplet paired state induced by Hund's rule coupling and correlations: a fully statistically consistent Gutzwiller approach.

    Science.gov (United States)

    Spałek, J; Zegrodnik, M

    2013-10-30

    The intrasite and intersite spin-triplet pairing gaps induced by interband Hund's rule coupling and their correlations are analyzed in the doubly degenerate Hubbard Hamiltonian. To include the effect of correlations, the statistically consistent Gutzwiller approximation is used. In this approach the consistency means that the averages calculated from the self-consistent equations and those determined variationally coincide with each other. Emphasis is put on the solution for which the average particle number is conserved when carrying out the Gutzwiller projection. This method leads to a stable equal-spin paired state in the so-called repulsive interactions limit (U > 3J) in the regime of moderate correlations. The interband hybridization introduces an inequivalence of the bands which, above a critical magnitude, suppresses the paired state due to both the Fermi-wavevector mismatch for the Cooper pair and the interband hopping allowed by the Pauli principle.

  20. Low-Spin Ferriheme Models of the Cytochromes: Correlation of Molecular Structure with EPR and Moessbauer Spectral Parameters

    Energy Technology Data Exchange (ETDEWEB)

    Teschner, T.; Trautwein, A. X.; Schuenemann, V. [University of Luebeck, Institute of Physics (Germany); Yatsunyk, L. A.; Walker, F. A. [University of Arizona, Department of Chemistry (United States)

    2004-12-15

    The magnetic Moessbauer spectra of a series of low-spin ferriheme complexes have been investigated and compared with their EPR spectral parameters and molecular structures. To date there has been little systematic analysis of either estimated or fitted values of the hyperfine coupling constants for low-spin ferriheme centers and no meaningful correlation has been established between the Moessbauer parameters and the axial ligands of such species. With the results of the present study, we have been able to find correlations of molecular structures with iron-orbital splittings, g-tensor values derived from EPR signals and magnetic hyperfine interaction components A{sub zz} obtained from magnetic Moessbauer spectra. These correlations should be useful to future workers in the field of heme-containing enzymes.

  1. Top Quark Polarization and Spin Correlation in the Littlest Higgs Model with T-Parity at the ILC

    Institute of Scientific and Technical Information of China (English)

    YANG Bing-Fang; LI Xiang-Dong

    2013-01-01

    In the framework of the littlest Higgs model with T-parity (LHT),we study the top quark spin correlation and polarization at the International Linear Collider (ILC).We find that the top quark polarization asymmetry δPt and the left-right asymmetry δALR car respectively reach-35% and-37.5% for √s =500 GeV and √s =1000 GeV via e+e-collision,which can reach the observable level at the ILC.By contrast,the spin correlation δC is smaller.The correlation behaviors of these observables at the e+ e-collision and the γγ collision will be helpful to distinguish different models and test the LHT model at the ILC.

  2. Muon Beam Tracking and Spin-Orbit Correlations for Precision g-2 Measurements

    Energy Technology Data Exchange (ETDEWEB)

    Tarazona, David [Michigan State U., East Lansing (main); Berz, Martin [Michigan State U., East Lansing (main); Hipple, Robert [Michigan State U., East Lansing (main); Makino, Kyoko [Michigan State U., East Lansing (main); Syphers, Michael [Fermilab

    2016-06-01

    The main goal of the Muon g-2 Experiment (g-2) at Fermilab is to measure the muon anomalous magnetic moment to unprecedented precision. This new measurement will allow to test the completeness of the Standard Model (SM) and to validate other theoretical models beyond the SM. The close interplay of the understanding of particle beam dynamics and the preparation of the beam properties with the experimental measurement is tantamount to the reduction of systematic errors in the determination of the muon anomalous magnetic moment. We describe progress in developing detailed calculations and modeling of the muon beam delivery system in order to obtain a better understanding of spin-orbit correlations, nonlinearities, and more realistic aspects that contribute to the systematic errors of the g-2 measurement. Our simulation is meant to provide statistical studies of error effects and quick analyses of running conditions for when g-2 is taking beam, among others. We are using COSY, a differential algebra solver developed at Michigan State University that will also serve as an alternative to compare results obtained by other simulation teams of the g-2 Collaboration.

  3. Reversible optical switching of antiferromagnetism in TbMnO3

    Science.gov (United States)

    Manz, Sebastian; Matsubara, Masakazu; Lottermoser, Thomas; Büchi, Jonathan; Iyama, Ayato; Kimura, Tsuyoshi; Meier, Dennis; Fiebig, Manfred

    2016-10-01

    Lasers can be used to control the magnetization of a ferromagnet via optically driven thermal and electronic excitation. Transfer of this concept to antiferromagnets is appealing because of the increasing technological interest in antiferromagnetism. Controlling spin structures in antiferromagnets is challenging, however, because of their zero magnetization. In a proof-of-principle experiment we demonstrate that optical control of antiferromagnetic domains is nevertheless possible. We reverse the antiferromagnetic order parameter in multiferroic TbMnO3 repeatedly, using light pulses of two different colours. Switching depends on a unique relation between the wavelength of the light, its optical absorption and the electric polarization field induced by the antiferromagnetic order of TbMnO3. We then demonstrate sequential laser-controlled writing and erasure of antiferromagnetic domains. The universality of reversible optical antiferromagnetic switching is derived by Monte Carlo simulations. Opto-magnetism is thus complemented by an important degree of freedom, namely local control of antiferromagnetism by means of light.

  4. Antiferromagnetic exchange mechanism of superconductivity in cuprates

    CERN Document Server

    Plakida, N M

    2001-01-01

    One examines theory of superconducting coupling resulted from antiferromagnetic exchange in terms of which one explains strong dependence of T sub c superconducting transition temperature on alpha lattice constant. Calculations are based on the Hubbard p-d two-region model within strong correlation limit. DELTA pd excitation high energy at antiferromagnetic exchange of two particles from different Hubbard subregions results in suppression o delay effects and in coupling of all particles in conductivity subregion with Fermi energy E sub F >= DELTA pd : T sub c approx = E sub F exp(-1/lambda), where lambda propor to J. T sub c (alpha) and isotopic effect are explained by J exchange interaction dependence on alpha and on zero oscillations of oxygen ions

  5. Unconventional normal-state spin dynamics in underdoped high-Tc cuprates as a fingerprint of spiral correlations of localized spins and dual localized/itinerant nature of spin fluctuations

    Science.gov (United States)

    Onufrieva, F.

    2017-03-01

    The paper is motivated by the observation of unusual and not well understood spin dynamics in low- and moderately doped high-Tc cuprates as well as by the discovery in these materials of a static incommensurate order for doping exceeding the insulator-metal boundary in the phase diagram. We develop a microscopic approach that allows us to treat accurately the quantum fluctuations in the spiral state developing upon doping the Mott-Neel insulator. We show that the spiral order of localized spins induces an off-diagonal order of mobile charges and a gap Δ ∝|Q | in their spectrum (Q is the spiral incommensurability wave vector defined with respect to QAF). Due to the dynamic spin-charge interaction the latter gap produces a feedback effect consisting in the appearence of a gap in the coherent spin excitation spectrum. As a result, the characteristic energy ωc=Δ appears, in the spin excitation spectra. It separates two components with qualitatively different behavior-above ωc, spin excitations are magnonlike and have an upward dispersion, below it, they are of the relaxation type and have a slight downward dispersion. The form of the dispersion is close to the form observed experimentally (by inelastic neutron scattering), which can be characterized as OPEN-hour-glass shaped or Y -shaped. There is no qualitative difference between the spin dynamics in the normal and SC states as far as doping is relatively low. There is no resonance. Other important features, including the incommensurability and uniaxial anisotropy of the low-energy spin excitations and the doping dependencies of the characteristic energy and wave vectors, are also close to those observed experimentally in low-doped cuprates. We show that the static spiral state becomes unstable at the critical doping nc. We show also that adopting the hypothesis about the presence of finite-energy spiral correlations in the paramagnetic state above nc and based on the results obtained for the static spiral state

  6. Effective Hamiltonian and low-lying eigenenergy clustering patterns of four-sublattice antiferromagnets

    DEFF Research Database (Denmark)

    Zhang, N.G.; Henley, C.L.; Rischel, C.;

    2002-01-01

    We study the low-lying eigenenergy clustering patterns of quantum antiferromagnets with p sublattices (in particular p = 4). We treat each sublattice as a large spin, and using second-order degenerate perturbation theory, we derive the effective (biquadratic) Hamiltonian coupling the p large spins....... In order to compare with exact diagonalizations, the Hamiltonian is explicitly written for a finite-size lattice, and it contains information on energies of excited states as well as the ground state. The result is applied to the face-centered-cubic Type-I antiferromagnet of spin 1/2, including second...

  7. HIGH-SPIN OCTUPOLE CORRELATIONS IN THE N=86, ND-146 AND SM-148 NUCLEI

    NARCIS (Netherlands)

    LIEDER, RM; BACELAR, JC; SINGH, PP; ALBER, D; BALABANSKI, D; GAST, W; GRAWE, H; HEBBINGHAUS, G; JONGMAN, [No Value; MOREK, T; NOORMAN, RF; RZACAURBAN, T; SCHNARE, H; THOMS, M; ZELL, O; NAZAREWICZ, W

    1991-01-01

    High-spin states in Nd-146 and Sm-148 have been populated using the C-13 + Xe-136 and Ne-22 + Te-130 compound nucleus reactions. Alternating parity bands built on the ground state are observed to spin I = (19) and I = (27) in Nd-146 and Sm-148 respectively. Analysis of the data done in terms of the

  8. Emergent spin-valley-orbital physics by spontaneous parity breaking

    Science.gov (United States)

    Hayami, Satoru; Kusunose, Hiroaki; Motome, Yukitoshi

    2016-10-01

    The spin-orbit coupling in the absence of spatial inversion symmetry plays an important role in realizing intriguing electronic states in solids, such as topological insulators and unconventional superconductivity. Usually, the inversion symmetry breaking is inherent in the lattice structures, and hence, it is not easy to control these interesting properties by external parameters. We here theoretically investigate the possibility of generating the spin-orbital entanglement by spontaneous electronic ordering caused by electron correlations. In particular, we focus on the centrosymmetric lattices with local asymmetry at the lattice sites, e.g. zigzag, honeycomb, and diamond structures. In such systems, conventional staggered orders, such as charge order and antiferromagnetic order, break the inversion symmetry and activate the antisymmetric spin-orbit coupling, which is hidden in a sublattice-dependent form in the paramagnetic state. Considering a minimal two-orbital model on a honeycomb structure, we scrutinize the explicit form of the antisymmetric spin-orbit coupling for all the possible staggered charge, spin, orbital, and spin-orbital orders. We show that the complete table is useful for understanding of spin-valley-orbital physics, such as spin and valley splitting in the electronic band structure and generalized magnetoelectric responses in not only spin but also orbital and spin-orbital channels, reflecting in peculiar magnetic, elastic, and optical properties in solids.

  9. Low-temperature Spin-Ice State of Quantum Heisenberg Magnets on Pyrochlore Lattice

    Science.gov (United States)

    Huang, Yuan; Chen, Kun; Deng, Youjin; Prokof'ev, Nikolay; Svistunov, Boris

    We establish that the isotropic spin-1/2 Heisenberg antiferromagnet on pyrochlore lattice enters a spin-ice state at low, but finite, temperature. Our conclusions are based on results of the bold diagrammatic Monte Carlo simulations that demonstrate good convergence of the skeleton series down to temperature T = J/6. The ``smoking gun'' identification of the spin-ice state is done through a remarkably accurate microscopic correspondence for static spin-spin correlation function between the quantum Heisenberg and classical Heisenberg/Ising models at all accessible temperatures. In particular, at T/J = 1/6, the momentum dependence shows a characteristic bow-tie pattern with pinch points. By numerical analytical continuation method, we also obtain the dynamic structure factor at real frequencies, showing a diffusive spinon dynamics at pinch points and spin wave continuum along the nodal lines.?

  10. Supersymmetry protected topological phases of isostatic lattices and kagome antiferromagnets

    Science.gov (United States)

    Lawler, Michael J.

    2016-10-01

    I generalize the theory of phonon topological band structures of isostatic lattices to frustrated antiferromagnets. I achieve this with a discovery of a many-body supersymmetry (SUSY) in the phonon problem of balls and springs and its connection to local constraints satisfied by ground states. The Witten index of the SUSY model demands the Maxwell-Calladine index of mechanical structures. "Spontaneous supersymmetry breaking" is identified as the need to gap all modes in the bulk to create the topological isostatic lattice state. Since ground states of magnetic systems also satisfy local constraint conditions (such as the vanishing of the total spin on a triangle), I identify a similar SUSY structure for many common models of antiferromagnets including the square, triangluar, kagome, pyrochlore nearest-neighbor antiferromagnets, and the J2=J1/2 square-lattice antiferromagnet. Remarkably, the kagome family of antiferromagnets is the analog of topological isostatic lattices among this collection of models. Thus, a solid-state realization of the theory of phonon topological band structure may be found in frustrated magnetic materials.

  11. Universality in antiferromagnetic strange metals

    Science.gov (United States)

    Maier, Stefan A.; Strack, Philipp

    2016-04-01

    We propose a theory of metals at the spin-density-wave quantum-critical point in spatial dimension d =2 . We provide a first estimate of the full set of critical exponents (dynamical exponent z =2.13 , correlation length ν =1.02 , spin susceptibility γ =0.96 , electronic non-Fermi liquid ητf=0.53 , spin-wave Landau damping ητb=1.06 ), which determine the universal power laws in thermodynamics and response functions in the quantum-critical regime relevant for experiments in heavy-fermion systems and iron pnictides. We present approximate numerical and analytical solutions of Polchinski-Wetterich-type flow equations with soft frequency regulators for an effective action of electrons coupled to spin-wave bosons. Performing the renormalization group in frequency instead of momentum space allows to track changes of the Fermi-surface shape and to capture Landau damping during the flow. The technique is easily generalizable from models retaining only patches of the Fermi surface to full, compact Fermi surfaces.

  12. The Andreev reflection in a superconductor-normal metal junction of a doped correlated quantum spin Hall insulator

    Science.gov (United States)

    Chang, Yung-Yeh; Mou, Chung-Yu; Chung, Chung-Hou

    Andreev conductance across a normal metal-superconductor (N-S) junction of doped correlated quantum spin Hall insulator on honeycomb lattice is theoretically studied via Blonder-Tinkham-Klapwijk (BTK) formalism. The normal side is modeled by the doped Kane-Mele (KM) model. The superconducting side is a doped correlated KM t-J model, which has been shown to feature d+id'-wave spin singlet pairing. With increasing intrinsic spin-orbit coupling, the doped KM t-J system undergoes a topological phase transition from the chiral d-wave superconductivity to the Z2 spin-Chern superconducting phase with helical Majorana fermions at edges. We apply a local strain on the N-S interface to generate an effective Dirac-delta barrier and study the transport near the chiral-helical phase transition in the weak tunneling limit. We explore the Andreev conductance at the K and K' Dirac points, respectively and find the distinctive behaviors across the transition. Relevance of our results for the adatom-doped graphene is discussed. Reference: S.J. Sun, C.H. Chung, Y.Y. Chang, W.F. Tsai, and F.C. Zhang, arXiv:1506.02584.'' Y.Y. C. acknowledges the support from the MOST Grant No.104-2112-M-009-004-MY3 and the NCTS of Taiwan, R.O.C.

  13. The peak effect (PE) region of the antiferromagnetic two layer Ising nanographene

    Energy Technology Data Exchange (ETDEWEB)

    Şarlı, Numan, E-mail: numansarli82@gmail.com [Institute of Science, Erciyes University, 38039 Kayseri (Turkey); Akbudak, Salih [Department of Physics, Adiyaman University, 02100 Adiyaman (Turkey); Department of Nanotechnology and Nanomedicine, Hacettepe University, 06800 Ankara (Turkey); Ellialtıoğlu, Mehmet Recai [Department of Physics Engineering, Hacettepe University, 06800 Ankara (Turkey)

    2014-11-01

    In this work, the magnetic properties of the ferromagnetic and antiferromagnetic two layer spin-1/2 Ising nanographene systems are investigated within the effective field theory. We find that the magnetizations and the hysteresis behaviors of the central graphene atoms are similar to those of the edge graphene atoms in the ferromagnetic case. But, they are quite different in the antiferromagnetic case. The antiferromagnetic central graphene atoms exhibit type II superconductivity and they have triple hysteresis loop. The peak effect (PE) region is observed on the hysteresis curves of the antiferromagnetic Ising nanographene system. Therefore, we suggest that there is a strong relationship between the antiferromagnetism and the peak effect. Our results are in agreement with some experimental works in recent literature.

  14. Half-metallic antiferromagnet as a prospective material for spintronics.

    Science.gov (United States)

    Hu, X

    2012-01-10

    Spintronics is expected as the next-generation technology based on the novel notch of spin degree of freedom of electrons. Half-metals, a class of materials which behave as a metal in one spin direction and an insulator in the opposite spin direction, are ideal for spintronic applications. Half-metallic antiferromagnets as a subclass of half-metals are characterized further by totally compensated spin moments in a unit cell, and have the advantage of being able to generate fully spin-polarized current while exhibiting zero macroscopic magnetization. Considerable efforts have been devoted to the search for this novel material, from which we may get useful insights for prospective material exploration.

  15. Antiferromagnetic vs. non-magnetic ε phase of solid oxygen. Periodic density functional theory studies using a localized atomic basis set and the role of exact exchange.

    Science.gov (United States)

    Ramírez-Solís, A; Zicovich-Wilson, C M; Hernández-Lamoneda, R; Ochoa-Calle, A J

    2017-01-25

    The question of the non-magnetic (NM) vs. antiferromagnetic (AF) nature of the ε phase of solid oxygen is a matter of great interest and continuing debate. In particular, it has been proposed that the ε phase is actually composed of two phases, a low-pressure AF ε1 phase and a higher pressure NM ε0 phase [Crespo et al., Proc. Natl. Acad. Sci. U. S. A., 2014, 111, 10427]. We address this problem through periodic spin-restricted and spin-polarized Kohn-Sham density functional theory calculations at pressures from 10 to 50 GPa using calibrated GGA and hybrid exchange-correlation functionals with Gaussian atomic basis sets. The two possible configurations for the antiferromagnetic (AF1 and AF2) coupling of the 0 ≤ S ≤ 1 O2 molecules in the (O2)4 unit cell were studied. Full enthalpy-driven geometry optimizations of the (O2)4 unit cells were done to study the pressure evolution of the enthalpy difference between the non-magnetic and both antiferromagnetic structures. We also address the evolution of structural parameters and the spin-per-molecule vs. pressure. We find that the spin-less solution becomes more stable than both AF structures above 50 GPa and, crucially, the spin-less solution yields lattice parameters in much better agreement with experimental data at all pressures than the AF structures. The optimized AF2 broken-symmetry structures lead to large errors of the a and b lattice parameters when compared with experiments. The results for the NM model are in much better agreement with the experimental data than those found for both AF models and are consistent with a completely non-magnetic (O2)4 unit cell for the low-pressure regime of the ε phase.

  16. Exchange biasing single molecule magnets: coupling of TbPc2 to antiferromagnetic layers.

    Science.gov (United States)

    Lodi Rizzini, A; Krull, C; Balashov, T; Mugarza, A; Nistor, C; Yakhou, F; Sessi, V; Klyatskaya, S; Ruben, M; Stepanow, S; Gambardella, P

    2012-11-14

    We investigate the possibility to induce exchange bias between single molecule magnets (SMM) and metallic or oxide antiferromagnetic substrates. Element-resolved X-ray magnetic circular dichroism measurements reveal, respectively, the presence and absence of unidirectional exchange anisotropy for TbPc(2) SMM deposited on antiferromagnetic Mn and CoO layers. TbPc(2) deposited on Mn thin films present magnetic hysteresis and a negative horizontal shift of the Tb magnetization loop after field cooling, consistent with the observation of pinned spins in the Mn layer coupled parallel to the Tb magnetic moment. Conversely, molecules deposited on CoO substrates present paramagnetic magnetization loops with no indication of exchange bias. These experiments demonstrate the ability of SMM to polarize the pinned uncompensated spins of an antiferromagnet during field-cooling and realize metal-organic exchange-biased heterostructures using antiferromagnetic pinning layers.

  17. The magnetoelectric properties study for system with the coexistence of the ferroelectric and antiferromagnetic orders

    Energy Technology Data Exchange (ETDEWEB)

    Jiang Qing; Zhong Chonggui

    2002-12-30

    Soft-mode theory based on DIFFOUR model for ferroelectric interaction and the mean-field theory of high spin Ising model for antiferromagnetic interaction are used to investigate the ferroelectric, antiferromagnetic, magnetoelectric properties in ferroelectromagnetic lattice in which the ferroelectric order and antiferromagnetic order coexist simultaneously below a certain temperature. Ferroelectric polarization, spin moment, and magnetoelectric susceptibility as well, as a function of temperature for system, are calculated and compared with the different coupling coefficient. It is found that an anomaly appears in curve of the polarization susceptibility as a function of temperature due to the coupling between the ferroelectric and antiferromagnetic orders in the ferroelectromagnetic lattice. At the same time, we also considered the influence of magnetoelectric effect on polarization susceptibility by applying the external field including electric and magnetic.

  18. Vector correlation analysis for inelastic and reactive collisions between partners possessing spin and orbital angular momentum.

    Science.gov (United States)

    Balint-Kurti, Gabriel G; Vasyutinskii, Oleg S

    2009-12-31

    A general reactive collision of the type A + B --> C + D is considered where both the collision partners (A and B) or the products (C and D) may possess internal, i.e., spin, orbital or rotational, angular momenta. Compact expressions are derived using a rigorous quantum mechanical analysis for the angular momentum anisotropy of either of the products (C or D) arising from an initially polarized distribution of the reactant angular momentum. The angular momentum distribution of the product is expressed in terms of canonical spherical tensors multiplied by anisotropy-transforming coefficients c(K(i)q(k))(K)(K(r),L). These coefficients act as transformation coefficients between the angular momentum anisotropy of the reactants and that of the product. They are independent of scattering angle but depend on the details of the scattering dynamics. The relationship between the coefficients c(K(i)q(k))(K)(K(r),L) and the body-fixed scattering S matrix is given and the methodology for the quantum mechanical calculation of the anisotropy-transforming coefficients is clearly laid out. The anisotropy-transforming coefficients are amenable to direct experimental measurement in a similar manner to vector correlation and alignment parameters in photodissociation processes. A key aspect of the theory is the use of projections of both reactant and product angular momenta onto the product recoil vector direction. An important new conservation rule is revealed through the analysis, namely that if the state multipole for reactant angular momentum distribution has a projection q(k) onto the product recoil vector the state multipoles for the product angular momentum distribution all have this same projection. Expressions are also presented for the distribution of the product angular momentum when its components are evaluated relative to the space-fixed Z-axis. Notes with detailed derivations of all the formulas are available as Supporting Information.

  19. Quantum discord in spin-cluster materials

    CERN Document Server

    Yurischev, M A

    2011-01-01

    The total quantum correlation (discord) in Heisenberg dimers is expressed via the spin-spin correlation function, internal energy, specific heat or magnetic susceptibility. This allows one to indirectly measure the discord through neutron scattering, as well as calorimetric or magnetometric experiments. Using the available experimental data, we found the discord for a number of binuclear Heisenberg substances with both antiferro- and ferromagnetic interactions. For the dimerized antiferromagnet copper nitrate Cu(NO_3)_2*2.5H_2O, the three independent experimental methods named above lead to a discord of approximately 0.2-0.3 bit/dimer at a temperature of 4 K. We also determined the temperature behavior of discord for hydrated and anhydrous copper acetates, as well as for the ferromagnetic binuclear copper acetate complex [Cu_2L(OAc)]*6H_2O, where L is a ligand.

  20. Resonating Valence Bond states for low dimensional S=1 antiferromagnets

    Science.gov (United States)

    Liu, Zheng-Xin; Zhou, Yi; Ng, Tai-Kai

    2014-03-01

    We study S = 1 spin liquid states in low dimensions. We show that the resonating-valence-bond (RVB) picture of S = 1 / 2 spin liquid state can be generalized to S = 1 case. For S = 1 system, a many-body singlet (with even site number) can be decomposed into superposition of products of two-body singlets. In other words, the product states of two-body singlets, called the singlet pair states (SPSs), are over complete to span the Hilbert space of many-body singlets. Furthermore, we generalized fermionic representation and the corresponding mean field theory and Gutzwiller projected stats to S = 1 models. We applied our theory to study 1D anti-ferromagnetic bilinear-biquadratic model and show that both the ground states (including the phase transition point) and the excited states can be understood excellently well within the framework. Our method can be applied to 2D S = 1 antiferromagnets.