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Sample records for americium 232

  1. Preparation of americium amalgam

    International Nuclear Information System (INIS)

    The authors describe a method for the electrochemical preparation of an americium amalgam from americium dioxide and americium 241 and 243 for use in determining the physicochemical properties of the alloy. Moessbauer spectra were made using neptunium dioxide, in the neptunium 237 form, as an absorber. Results show that electrolysis produces a homogeneous amalgam that gives an unoxidized product on vacuum distillation at 200 degrees C

  2. Preparation of americium amalgam

    International Nuclear Information System (INIS)

    Using the method of NGR-spectroscopy with the aid of 241Am isotope chemical state of transuranium elements in the volume and on the surface of amalgams is studied. Amalgam preparation was realized in a simplified electrolytic cell. It is shown that in the process of amalgam preparation the first order of reaction as to actinide is observed; americium is distributed gradually over the volume and it is partially sorbed by the surface of glass capillary. NGR spectrum of dry residue after mercury distillation at 200 deg C points to the presence of americium-mercury intermetal compounds

  3. 1976 Hanford americium accident

    Energy Technology Data Exchange (ETDEWEB)

    Heid, K R; Breitenstein, B D; Palmer, H E; McMurray, B J; Wald, N

    1979-01-01

    This report presents the 2.5-year medical course of a 64-year-old Hanford nuclear chemical operator who was involved in an accident in an americium recovery facility in August 1976. He was heavily externally contaminated with americium, sustained a substantial internal deposition of this isotope, and was burned with concentrated nitric acid and injured by flying debris about the face and neck. The medical care given the patient, including the decontamination efforts and clinical laboratory studies, are discussed. In-vivo measurements were used to estimate the dose rates and the accumulated doses to body organs. Urinary and fecal excreta were collected and analyzed for americium content. Interpretation of these data was complicated by the fact that the intake resulted both from inhalation and from solubilization of the americium embedded in facial tissues. A total of 1100 ..mu..Ci was excreted in urine and feces during the first 2 years following the accident. The long-term use of diethylenetriaminepentate (DTPA), used principally as the zinc salt, is discussed including the method, route of administration, and effectiveness. To date, the patient has apparently experienced no complications attributable to this extensive course of therapy, even though he has been given approximately 560 grams of DTPA. 4 figures, 1 table.

  4. Chemistry of americium

    Energy Technology Data Exchange (ETDEWEB)

    Schulz, W.W.

    1976-01-01

    Essential features of the descriptive chemistry of americium are reviewed. Chapter titles are: discovery, atomic and nuclear properties, collateral reading, production and uses, chemistry in aqueous solution, metal, alloys, and compounds, and, recovery, separation, purification. Author and subject indexes are included. (JCB)

  5. The Biokinetic Model of Americium

    Institute of Scientific and Technical Information of China (English)

    2011-01-01

    To improve in vivo measurements for detecting internal exposure from transuranium radio nuclides, such as neptunium, plutonium, americium, the bioknetic model was studied. According to ICRP report (1993, 1995, 1997) and other research, the

  6. Americium product solidification and disposal

    International Nuclear Information System (INIS)

    The americium product from the TRUEX processing plant needs to be converted into a form suitable for ultimate disposal. An evaluation of the disposal based on safety, number of process steps, demonstrated operability of the processes, production of low-level alpha waste streams, and simplicity of maintenance with low radiation exposures to personnel during maintenance, has been made. The best process is to load the americium on a cation exchange resin followed by calcination or oxidation of the resin after loading

  7. 17 CFR 232.403-232.404 - [Reserved

    Science.gov (United States)

    2010-04-01

    ... 17 Commodity and Securities Exchanges 2 2010-04-01 2010-04-01 false 232.403-232.404 Section 232.403-232.404 Commodity and Securities Exchanges SECURITIES AND EXCHANGE COMMISSION REGULATION S-T-GENERAL RULES AND REGULATIONS FOR ELECTRONIC FILINGS Xbrl-Related Documents §§ 232.403-232.404...

  8. Spectrochemical analysis of curium and americium samples

    International Nuclear Information System (INIS)

    Spectrochemical procedures have been developed to determine impurities in americium and curium samples. The simultaneous separation of many impurity elements from the base material (americium and curium) is carried out with extraction and extraction-chromatographic methods using di-2-ethylhexylphosphoric acid. It is shown that part of the elements are separated with extraction or sorption of americium and curium; the other part with the Talspeak process. Two fractions in the extraction chromatography and three fractions in the extraction separation of americium and curium, containing impurities, are analyzed separately by a.c. or d.c. arc spectrography. To increase the sensitivity of the spectrographic analysis and accelerate the burn-up of impurities from the crater of the carbon electrode bismuth fluoride and sodium chloride were used as chemically active substances. The extraction of impurities from weighed quantities of americium and curium samples of 5 to 10 mg permits the lower limit of determined impurity concentrations to be extended to 1 x 10-4 to 5 x 10-3% m/m. (author)

  9. Pyrochemical technology of plutonium and americium preparation and purification

    International Nuclear Information System (INIS)

    Pyrochemical tecnology of metallic plutonium and americium preparation and purification is considered. Investigations into plutonium dioxide reduction up to metal; plutonium electrolytic refining in molten salts; plutonium extraction from the molten salts and preparation of americium dioxide and metallic americium from its tetrafluoride are described

  10. Aqueous Chloride Operations Overview: Plutonium and Americium Purification/Recovery

    Energy Technology Data Exchange (ETDEWEB)

    Kimball, David Bryan [Los Alamos National Lab. (LANL), Los Alamos, NM (United States); Skidmore, Bradley Evan [Los Alamos National Lab. (LANL), Los Alamos, NM (United States)

    2016-06-22

    Acqueous Chloride mission is to recover plutonium and americium from pyrochemical residues (undesirable form for utilization and storage) and generate plutonium oxide and americium oxide. Plutonium oxide is recycled into Pu metal production flowsheet. It is suitable for storage. Americium oxide is a valuable product, sold through the DOE-OS isotope sales program.

  11. 1976 Hanford americium exposure incident: psychological aspects

    International Nuclear Information System (INIS)

    Accidents involving exposure to radiation or radioactive materials may involve an unusual degree of emotional trauma. Methods that may be employed in dealing with such trauma are discussed in relation to a specific accident in which a radiation worker was injured and seriously contaminated with americium-241

  12. RS-232 Led Board

    CERN Document Server

    Tskhvaradze, Vladimir

    2007-01-01

    This article demonstrates how to develop a Microchip PIC16F84 based device that supports RS-232 interface with PC. Circuit (LED Board) design and software development will be discussed. PicBasic Pro Compiler from microEngineering Labs, Inc. is used for PIC programming. Development of LED Board Control Console using C/C++ is also briefly discussed. The project requires basic work experience with Microchip PICs, serial communication and programming.

  13. Incentives for transmutation of americium in thermal reactors

    International Nuclear Information System (INIS)

    This report describes possible benefits when americium is irradiated in a thermal reactor. If all plutonium is partitioned from spent fuel, americium is the main contributor to the radiotoxicity of spent fuel upto several thousands of years of storage. It is shown that americium can be transmuted to other nuclides upon irradiation in a thermal reactor, leading to a 50% reduction of the radiotoxicity of neptunium, which can be an important contributor to the dose due to leakage of nuclides after one million years of storage. The radiotoxicity of americium can be reduced considerably after irradiation for 3 to 6 years in a thermal reactor with thermal neutron flux of 1014 cm-2s-1. The strongly α and neutron emitting transmutation products can most probably not be recycled again, so a transmutation process is suggested in which americium is irradiated for 3 to 6 years and then put to final storage. It is shown that the radiotoxicity of the transmuation products after a storage time of about one hundred years can be considerably reduced compared to the radiotoxicity of the initial americium. The same holds for the α activity and heat emission of the transmutation products. Because plutonium in spent fuel contributes for about 80% to the radiotoxicity upto 105 years of storage, recycling and transmutation of plutonium has first priority. Transmutation of americium is only meaningful when the radiotoxicity of plutonium is reduced far below the radiotoxicity of americium. (orig.)

  14. Surface complexation modeling of americium sorption onto volcanic tuff.

    Science.gov (United States)

    Ding, M; Kelkar, S; Meijer, A

    2014-10-01

    Results of a surface complexation model (SCM) for americium sorption on volcanic rocks (devitrified and zeolitic tuff) are presented. The model was developed using PHREEQC and based on laboratory data for americium sorption on quartz. Available data for sorption of americium on quartz as a function of pH in dilute groundwater can be modeled with two surface reactions involving an americium sulfate and an americium carbonate complex. It was assumed in applying the model to volcanic rocks from Yucca Mountain, that the surface properties of volcanic rocks can be represented by a quartz surface. Using groundwaters compositionally representative of Yucca Mountain, americium sorption distribution coefficient (Kd, L/Kg) values were calculated as function of pH. These Kd values are close to the experimentally determined Kd values for americium sorption on volcanic rocks, decreasing with increasing pH in the pH range from 7 to 9. The surface complexation constants, derived in this study, allow prediction of sorption of americium in a natural complex system, taking into account the inherent uncertainty associated with geochemical conditions that occur along transport pathways.

  15. Electrochemical oxidation of americium in nitric medium: study of reaction mechanisms; Oxydation de l'americium par voie electrochimique: etude des mecanismes

    Energy Technology Data Exchange (ETDEWEB)

    Picart, S.; Chartier, D.; Donnet, L.; Adnet, J.M. [CEA Valrho, (DCC/DRRV/SPHA), 30 - Marcoule (France)

    2000-07-01

    One alternative selected by the CEA for partitioning minor actinides from aqueous solutions containing fission products is the selective extraction of oxidized americium. This is the SESAME process (Selective Extraction and Separation of Americium by Means of Electrolysis) aimed to convert americium to oxidation state (VI) and then extract it with a specific extractant of high valences. This paper presents the study of the electrochemical oxidation of americium in nitric medium which represents an important stage of the process. The reaction can be divided into two main steps: oxidation of americium (III) to americium (IV), and then of americium (IV) to americium (VI). For the first oxidation step, a ligand L is needed to stabilize the intermediate species americium (IV) which disproportionates in its free form into americium (III) and (V). Phospho-tungstate or silico-tungstate are appropriate ligands because they are stable in concentrated nitric acid and show a great affinity for metallic cations at oxidation state (IV) (Table 1 lists the stability constants of americium (IV) complexes). The presence of the lacunary poly-anion lowers the potential of the americium (IV) / americium (Ill) redox pair (see Figure 5 for the diagram of the apparent formal potential of americium versus ligand concentration). This makes it thermodynamically possible to oxidize americium (III) into americium (IV) at the anode of an electrolyzer in nitric acid. For the second oxidation step, a strong oxidant redox mediator, like silver (II), is needed to convert complexed americium at oxidation state (IV) to oxidation state (V). The AmVL complex is then hydrolyzed to yield americyle (V) aqua ion. A spectroscopic Raman study with {sup 18}O labeled species showed that the oxygen atoms of the americyle moiety came from water. This indicates that water hydrolyzes the americium (V) complex to produce americyle (V) aqua ion, AmO{sub 2}{sup +}. This cation reacts with silver (Il) to give

  16. 17 CFR 232.10 - Application of part 232.

    Science.gov (United States)

    2010-04-01

    ... within two business days before or after the electronic Form ID filing, a notarized document, manually...-T-GENERAL RULES AND REGULATIONS FOR ELECTRONIC FILINGS General § 232.10 Application of part 232. (a) This part, in conjunction with the EDGAR Filer Manual and the electronic filing provisions...

  17. Higher Americium Oxidation State Research Roadmap

    Energy Technology Data Exchange (ETDEWEB)

    Mincher, Bruce J. [Idaho National Lab. (INL), Idaho Falls, ID (United States); Law, Jack D. [Idaho National Lab. (INL), Idaho Falls, ID (United States); Goff, George S. [Los Alamos National Lab. (LANL), Los Alamos, NM (United States); Moyer, Bruce A. [Oak Ridge National Lab. (ORNL), Oak Ridge, TN (United States); Burns, Jon D. [Oak Ridge National Lab. (ORNL), Oak Ridge, TN (United States); Lumetta, Gregg J. [Pacific Northwest National Lab. (PNNL), Richland, WA (United States); Sinkov, Sergey I. [Pacific Northwest National Lab. (PNNL), Richland, WA (United States); Shehee, Thomas C. [Savannah River Site (SRS), Aiken, SC (United States). Savannah River National Lab. (SRNL); Hobbs, David T. [Savannah River Site (SRS), Aiken, SC (United States). Savannah River National Lab. (SRNL)

    2015-12-18

    The partitioning of hexavalent Am from dissolved nuclear fuel requires the ability to efficiently oxidize Am(III) to Am(VI) and to maintain that oxidation state for a length of time sufficient to perform the separation. Several oxidants have been, or are being developed. Chemical oxidants include Ag-catalyzed ozone, Ag-catalyzed peroxydisulfate, Cu(III) periodate, and sodium bismuthate. Hexavalent americium has also now successfully been prepared by electrolysis, using functionalized electrodes. So-called auto-reduction rates of Am(VI) are sufficiently slow to allow for separations. However, for separations based on solvent extraction or ion exchange using organic resins, the high valence state must be maintained under the reducing conditions of the organic phase contact, and a holding oxidant is probably necessary. Until now, only Cu(III) periodate and sodium bismuthate oxidation have been successfully combined with solvent extraction separations. Bismuthate oxidation provided the higher DAm, since it acts as its own holding oxidant, and a successful hot test using centrifugal contactors was performed. For the other oxidants, Ag-catalyzed peroxydisulfate will not oxidize americium in nitric acid concentrations above 0.3 M, and it is not being further investigated. Peroxydisulfate in the absence of Ag catalysis is being used to prepare Am(V) in ion exchange work, discussed below. Preliminary work with Ag-catalyzed ozone has been unsuccessful for extractions of Am(VI) from 6.5 M HNO3, and only one attempt at extraction, also from 6.5 M HNO3, using the electrolytic oxidation has been attempted. However, this high acid concentration was based on the highest Am extraction efficiency using the bismuthate oxidant; which is only sparingly soluble, and thus the oxidation yield is based on bismuthate solubility. Lower acid concentrations may be sufficient with alternative oxidants and work with Ag-ozone, Cu(III) and electrolysis is on-going. Two non

  18. Plutonium and Americium Geochemistry at Hanford: A Site Wide Review

    Energy Technology Data Exchange (ETDEWEB)

    Cantrell, Kirk J.; Felmy, Andrew R.

    2012-08-23

    This report was produced to provide a systematic review of the state-of-knowledge of plutonium and americium geochemistry at the Hanford Site. The report integrates existing knowledge of the subsurface migration behavior of plutonium and americium at the Hanford Site with available information in the scientific literature regarding the geochemistry of plutonium and americium in systems that are environmentally relevant to the Hanford Site. As a part of the report, key research needs are identified and prioritized, with the ultimate goal of developing a science-based capability to quantitatively assess risk at sites contaminated with plutonium and americium at the Hanford Site and the impact of remediation technologies and closure strategies.

  19. Mixed chelation therapy for removal of plutonium and americium

    International Nuclear Information System (INIS)

    Iron-binding compounds, 2,3-dihydroxybenzoic acid (DHBA), 2-hydroxybenzoic acid (HBA), and 2-(acetyloxy)benzoic acid (ABA), were tested for their ability to remove americium and plutonium from rats following intraperitioneal injection of the radionuclides as citrates (pH 5). Treatments, 2 mmol/kg, were given on days 3, 6, 10, 12 and 14 following the actinide injection. DHBA and HBA caused about a 20% decrease in liver retention of americium compared to the control value, and DHB caused a similar effect for plutonium. The above agents, co-administered with 0.5 mmol polyaminopolycarboxylic acid (PAPCA)-type chelons, did not change tissue retention of americium and plutonium from that due to the PAPCAs alone. Administration of americium and plutonium to the same rats is useful for studying removal agents since the two actinides behave independently in their biological disposition and response to removal

  20. Gamma-sources on the basis of metallic americium-241

    International Nuclear Information System (INIS)

    A batch of gamma-radiation sources has been manufactured from metallic americium-241 of isotopic purity, its activity varying from 0.08 to 0.93 GBq. The cores of the sources are high-purity americium metal condensate on a tantalum or stainless steel substrate prepared by thermal decomposition of 241Pu-241Am alloy in a high vacuum. 7 refs., 1 tab

  1. Aqueous Chloride Operations Overview: Plutonium and Americium Purification/Recovery

    Energy Technology Data Exchange (ETDEWEB)

    Gardner, Kyle Shelton [Los Alamos National Lab. (LANL), Los Alamos, NM (United States); Kimball, David Bryan [Los Alamos National Lab. (LANL), Los Alamos, NM (United States); Skidmore, Bradley Evan [Los Alamos National Lab. (LANL), Los Alamos, NM (United States)

    2016-09-28

    These are a set of slides intended for an information session as part of recruiting activities at Brigham Young University. It gives an overview of aqueous chloride operations, specifically on plutonium and americium purification/recovery. This presentation details the steps taken perform these processes, from plutonium size reduction, dissolution, solvent extraction, oxalate precipitation, to calcination. For Americium recovery, it details the CLEAR (chloride extraction and actinide recovery) Line, oxalate precipitation and calcination.

  2. Pyrochemical investigations into recovering plutonium from americium extraction salt residues

    International Nuclear Information System (INIS)

    Progress into developing a pyrochemical technique for separating and recovering plutonium from spent americium extraction waste salts has concentrated on selective chemical reduction with lanthanum metal and calcium metal and on the solvent extraction of americium with calcium metal. Both techniques are effective for recovering plutonium from the waste salt, although neither appears suitable as a separation technique for recycling a plutonium stream back to mainline purification processes. 17 refs., 13 figs., 2 tabs

  3. A study of the generation of 232U in UO2 and MOX fuels

    International Nuclear Information System (INIS)

    To clarify the generation pathway of 232U, an important nuclide for dose evaluation at various stages in the reuse of uranium, concentrations of 232U generated through various pathways were evaluated for UO2 and mixed oxide (MOX) fuels. Burnup calculation was conducted with ORIGEN2.2 code adopting ORLIBJ40 library, a set of cross-section libraries based on JENDL-4.0. It was found that differences in 232U concentrations in UO2 and MOX fuels mainly arise from differences in the initial compositions of 234U, 235U, and 236U. It was also found that the contribution of plutonium and americium isotopes in MOX fuels is small compared with that of uranium isotopes. The results clarified that the capture cross sections of 230Th, 231Pa, 235U, and 236U, as well as the (n,2n) cross sections of 237Np and 238U, have a large effect on the generation of 232U. Additional investigation showed that 232U concentration is strongly affected not only by time after irradiation but also by time before irradiation. (author)

  4. Electrochemical oxidation of americium in nitric medium: study of reaction mechanisms

    International Nuclear Information System (INIS)

    One alternative selected by the CEA for partitioning minor actinides from aqueous solutions containing fission products is the selective extraction of oxidized americium. This is the SESAME process (Selective Extraction and Separation of Americium by Means of Electrolysis) aimed to convert americium to oxidation state (VI) and then extract it with a specific extractant of high valences. This paper presents the study of the electrochemical oxidation of americium in nitric medium which represents an important stage of the process. The reaction can be divided into two main steps: oxidation of americium (III) to americium (IV), and then of americium (IV) to americium (VI). For the first oxidation step, a ligand L is needed to stabilize the intermediate species americium (IV) which disproportionates in its free form into americium (III) and (V). Phospho-tungstate or silico-tungstate are appropriate ligands because they are stable in concentrated nitric acid and show a great affinity for metallic cations at oxidation state (IV) (Table 1 lists the stability constants of americium (IV) complexes). The presence of the lacunary poly-anion lowers the potential of the americium (IV) / americium (Ill) redox pair (see Figure 5 for the diagram of the apparent formal potential of americium versus ligand concentration). This makes it thermodynamically possible to oxidize americium (III) into americium (IV) at the anode of an electrolyzer in nitric acid. For the second oxidation step, a strong oxidant redox mediator, like silver (II), is needed to convert complexed americium at oxidation state (IV) to oxidation state (V). The AmVL complex is then hydrolyzed to yield americyle (V) aqua ion. A spectroscopic Raman study with 18O labeled species showed that the oxygen atoms of the americyle moiety came from water. This indicates that water hydrolyzes the americium (V) complex to produce americyle (V) aqua ion, AmO2+. This cation reacts with silver (Il) to give americyle (VI) ion. Figure

  5. Applicability of insoluble tannin to treatment of waste containing americium

    International Nuclear Information System (INIS)

    The applicability of insoluble tannin adsorbent to the treatment of aqueous waste contaminated with americium has been investigated. Insoluble tannin is considered highly applicable because it consists of only carbon, hydrogen and oxygen and so its volume can be easily reduced by incineration. This report describes measurements of the americium distribution coefficient in low concentration nitric acid. The americium distribution coefficients were found to decrease with increasing concentration of nitric acid and sodium nitrate, and with increasing temperature. At 25 C in 2.0 x 10-3 M HNO3, the distribution coefficient was found to be 2000 ml g-1. The adsorption capacity was determined by column experiments using europium as a simulant of americium, and found to be 7 x 10-3 mmol g-1-dried tannin in 0.01 M HNO3 at 25 C, which corresponds to approximately 1.7 mg-241Am/g-adsorbent(dried). The prospect of applying the adsorbent to the treatment of aqueous waste contaminated with americium appears promising. (orig.)

  6. Salvage of plutonium-and americium-contaminated metals

    International Nuclear Information System (INIS)

    Melt-slagging techniques were evaluated as a decontamination and consolidation step for metals contaminated with oxides of plutonium and americium. Experiments were performed in which mild steel, stainless steel, and nickel metals contaminated with oxides of plutonium and americium were melted in the presence of silicate slags of various compositions. The metal products were low in contamination, with the plutonium and americium strongly fractionated to the slags. Partition coefficients (plutonium in slag/plutonium in steel) of 7*10/sup 6/ with borosilicate slag and 3*10/sup 6/ for calcium, magnesium silicate slag were measured. Decontamination of metals containing as much as 14,000 p.p.m. plutonium appears to be as efficient as that of metals with plutonium levels of 400 p.p.m. Staged extraction, that is, a remelting of processed metal with clean slag, results in further decontamination of the metal. 10 refs

  7. 1976 Hanford americium exposure incident: overview and perspective

    International Nuclear Information System (INIS)

    Salient features of the 1976 Hanford americium exposure incident are discussed. Comparisons are made with previous human and animal exposure data, and conclusions drawn relative to the injured workman, to health physics practices, and to the adequacy of current exposure limits

  8. 232Th, a rigid rotor

    International Nuclear Information System (INIS)

    We undertake the present work to treat 232Th with a soft rotor formula used recently by C. Bihari et. al for γ-band and modified by J.B. Gupta et. al. It describes energy in terms of moment of inertia and softness parameter

  9. Reduction Rates for Higher Americium Oxidation States in Nitric Acid

    Energy Technology Data Exchange (ETDEWEB)

    Grimes, Travis Shane [Idaho National Lab. (INL), Idaho Falls, ID (United States); Mincher, Bruce Jay [Idaho National Lab. (INL), Idaho Falls, ID (United States); Schmitt, Nicholas C [Idaho National Lab. (INL), Idaho Falls, ID (United States)

    2015-09-30

    The stability of hexavalent americium was measured using multiple americium concentrations and nitric acid concentrations after contact with the strong oxidant sodium bismuthate. Contrary to our hypotheses Am(VI) was not reduced faster at higher americium concentrations, and the reduction was only zero-order at short time scales. Attempts to model the reduction kinetics using zero order kinetic models showed Am(VI) reduction in nitric acid is more complex than the autoreduction processes reported by others in perchloric acid. The classical zero-order reduction of Am(VI) was found here only for short times on the order of a few hours. We did show that the rate of Am(V) production was less than the rate of Am(VI) reduction, indicating that some Am(VI) undergoes two electron-reduction to Am(IV). We also monitored the Am(VI) reduction in contact with the organic diluent dodecane. A direct comparison of these results with those in the absence of the organic diluent showed the reduction rates for Am(VI) were not statistically different for both systems. Additional americium oxidations conducted in the presence of Ce(IV)/Ce(III) ions showed that Am(VI) is reduced without the typical growth of Am(V) observed in the systems sans Ce ion. This was an interesting result which suggests a potential new reduction/oxidation pathway for Am in the presence of Ce; however, these results were very preliminary, and will require additional experiments to understand the mechanism by which this occurs. Overall, these studies have shown that hexavalent americium is fundamentally stable enough in nitric acid to run a separations process. However, the complicated nature of the reduction pathways based on the system components is far from being rigorously understood.

  10. Synthesis and characterization of uranium-americium mixed oxides

    International Nuclear Information System (INIS)

    Americium isotopes represent a significant part of high-level and long-lived nuclear waste in spent fuels. Among the envisaged reprocessing scenarios, their transmutation in fast neutron reactors using uranium-americium mixed-oxide pellets (U1-xAmxO2±δ) is a promising option which would help decrease the ecological footprint of ultimate waste repository sites. In this context, this thesis is dedicated to the study of such compounds over a wide range of americium contents (7.5 at.% ≤ Am/(U+Am) ≤ 70 at.%), with an emphasis on their fabrication from single-oxide precursors and the assessment of their structural and thermodynamic stabilities, also taking self-irradiation effects into account. Results highlight the main influence of americium reduction to Am(+III), not only on the mechanisms of solid-state formation of the U1-xAmxO2±δ solid solution, but also on the stabilization of oxidized uranium cations and the formation of defects in the oxygen sublattice such as vacancies and cub-octahedral clusters. In addition, the data acquired concerning the stability of U1-xAmxO2±δ compounds (existence of a miscibility gap, vaporization behavior) were compared to calculations based on new thermodynamic modelling of the U-Am-O ternary system. Finally, α-self-irradiation-induced structural effects on U1-xAmxO2±δ compounds were analyzed using XRD, XAS and TEM, allowing the influence of americium content on the structural swelling to be studied as well as the description of the evolution of radiation-induced structural defects. (author)

  11. 48 CFR 232.616 - Compromise actions.

    Science.gov (United States)

    2010-10-01

    ..., DEPARTMENT OF DEFENSE GENERAL CONTRACTING REQUIREMENTS CONTRACT FINANCING Contract Debts 232.616 Compromise actions. Only the department/agency contract financing offices (see 232.070(c)) are authorized...

  12. 49 CFR 232.611 - Periodic maintenance.

    Science.gov (United States)

    2010-10-01

    ... 49 Transportation 4 2010-10-01 2010-10-01 false Periodic maintenance. 232.611 Section 232.611 Transportation Other Regulations Relating to Transportation (Continued) FEDERAL RAILROAD ADMINISTRATION... maintenance. (a) In addition to the maintenance requirements contained in § 232.303(b) through (d), a...

  13. 8 CFR 232.3 - Arriving aliens.

    Science.gov (United States)

    2010-01-01

    ... 8 Aliens and Nationality 1 2010-01-01 2010-01-01 false Arriving aliens. 232.3 Section 232.3 Aliens and Nationality DEPARTMENT OF HOMELAND SECURITY IMMIGRATION REGULATIONS DETENTION OF ALIENS FOR PHYSICAL AND MENTAL EXAMINATION § 232.3 Arriving aliens. When a district director has reasonable...

  14. 7 CFR 58.232 - Milk.

    Science.gov (United States)

    2010-01-01

    ... 7 Agriculture 3 2010-01-01 2010-01-01 false Milk. 58.232 Section 58.232 Agriculture Regulations of the Department of Agriculture (Continued) AGRICULTURAL MARKETING SERVICE (Standards, Inspections....232 Milk. Raw milk shall meet the requirements as outlined in §§ 58.132 through 58.138 and,...

  15. 24 CFR 232.3 - Bathroom.

    Science.gov (United States)

    2010-04-01

    ... 24 Housing and Urban Development 2 2010-04-01 2010-04-01 false Bathroom. 232.3 Section 232.3... Eligibility Requirements § 232.3 Bathroom. Not less than one full bathroom must be provided for every four residents of a board and care home or assisted living facility, and bathroom access from any bedroom...

  16. Neptunium and americium control for international non-proliferation regime

    International Nuclear Information System (INIS)

    It was decided in the IAEA Board of Governors Meeting held in Sept. 1999 that Neptunium and Americium could be diverted for manufacturing nuclear weapon or explosives, so that appropriate measures should be taken for the prevention of proliferation of these materials. It is expected to take relatively long time for settling down the aligned system dealing with the above materials because the present regulatory statement was prepared on the basis of voluntary offers from the States concerned. The necessity of preventive measures is being convinced among Member States, but it would not be easy to take voluntary participation in detail because of their respective interests. It is expected that this paper could contribute to the effective response as to the international commitments as well as for protecting the domestic nuclear industry and R and D area through analysis on the IAEA's approach on Neptunium and Americium

  17. Thermophysical properties of americium-containing barium plutonate

    International Nuclear Information System (INIS)

    Polycrystalline specimens of americium-containing barium plutonate have been prepared by mixing the appropriate amounts of (Pu0.91Am0.09)O2 and BaCO3 powders followed by reacting and sintering at 1600 K under the flowing gas atmosphere of dry-air. The sintered specimens had a single phase of orthorhombic perovskite structure and were crack-free. Elastic moduli were determined from longitudinal and shear sound velocities. Debye temperature was also determined from sound velocities and lattice parameter measurements. Thermal conductivity was calculated from measured density at room temperature, literature values of heat capacity and thermal diffusivity measured by laser flash method in vacuum. Thermal conductivity of americium-containing barium plutonate was roughly independent of temperature and registered almost the same magnitude as that of BaPuO3 and BaUO3. (author)

  18. 1976 Hanford americium-exposure incident: decontamination and treatment facility

    International Nuclear Information System (INIS)

    An injured worker, contaminated with over 6 mCi of americium-241, required special treatment and housing for 4 months. This paper is a description of the design and management of the facility in which most of the treatment and housing occurred. The problems associated with contamination control, waste handling, supplies, and radiological concerns during the two-stage transfer of the patient from a controlled situation to his normal living environment are discussed in detail

  19. Ingestion Pathway Transfer Factors for Plutonium and Americium

    Energy Technology Data Exchange (ETDEWEB)

    Blanchard, A.

    1999-07-28

    Overall transfer factors for major ingestion pathways are derived for plutonium and americium. These transfer factors relate the radionuclide concentration in a given foodstuff to deposition on the soil. Equations describing basic relationships consistent with Regulatory Guide 1.109 are followed. Updated values and coefficients from IAEA Technical Reports Series No. 364 are used when a available. Preference is given to using factors specific to the Savannah River Site.

  20. Method for removal of plutonium impurity from americium oxides and fluorides

    Science.gov (United States)

    FitzPatrick, John R.; Dunn, Jerry G.; Avens, Larry R.

    1987-01-01

    Method for removal of plutonium impurity from americium oxides and fluorides. AmF.sub.4 is not further oxidized to AmF.sub.6 by the application of O.sub.2 F at room temperature, while plutonium compounds present in the americium sample are fluorinated to volatile PuF.sub.6, which can readily be separated therefrom, leaving the purified americium oxides and/or fluorides as the solid tetrafluoride.

  1. Gut uptake factors for plutonium, americium and curium

    International Nuclear Information System (INIS)

    Data on estimates of the absorption of plutonium, americium and curium from the human gut based on measurements of uptake in other mammalian species are reviewed. It is proposed that for all adult members of the public ingesting low concentrations of plutonium in food and water, 0.05% would be an appropriate value of absorption except when the conditions of exposure are known and a lower value can be justified. For dietary intakes of americium and curium, the available data do not warrant a change from the ICRP value of 0.05%. For newborn children ingesting americium, curium and soluble forms of plutonium, a value of 1% absorption is proposed for the first 3 months of life during which the infant is maintained on a milk diet. It is proposed that a value of 0.5% should be used for the first year of life to take account of the gradual maturation of the gut. In considering the ingestion of insoluble oxides of plutonium by infants, it is proposed that absorption is taken as 0.1% for the first 3 months and 0.05% for the first year. (author)

  2. Network Coding Over The 232

    DEFF Research Database (Denmark)

    Pedersen, Morten Videbæk; Heide, Janus; Vingelmann, Peter;

    2013-01-01

    Creating efficient finite field implementations has been an active research topic for several decades. Many appli- cations in areas such as cryptography, signal processing, erasure coding and now also network coding depend on this research to deliver satisfactory performance. In this paper we...... investigate the use of prime fields with a field size of 232 − 5, as this allows implementations which combines high field sizes and low complexity. First we introduce the algorithms needed to apply prime field arithmetics to arbitrary binary data. After this we present the initial throughput measurements...... will be useful in many network coding applications where large field sizes are required....

  3. 17 CFR 232.11 - Definition of terms used in part 232.

    Science.gov (United States)

    2010-04-01

    ... information in eXtensible Business Reporting Language (XBRL) electronic format pursuant to § 232.405... Rule 104 of Regulation S-T (§ 232.104). XBRL-Related Documents. The term XBRL-Related Documents...

  4. Airborne plutonium-239 and americium-241 concentrations measured from the 125-meter Hanford Meteorological Tower

    International Nuclear Information System (INIS)

    Airborne plutonium-239 and americium-241 concentrations and fluxes were measured at six heights from 1.9 to 122 m on the Hanford meteorological tower. The data show that plutonium-239 was transported on nonrespirable and small particles at all heights. Airborne americium-241 concentrations on small particles were maximum at the 91 m height

  5. 10 CFR 31.8 - Americium-241 and radium-226 in the form of calibration or reference sources.

    Science.gov (United States)

    2010-01-01

    ... 10 Energy 1 2010-01-01 2010-01-01 false Americium-241 and radium-226 in the form of calibration or... BYPRODUCT MATERIAL § 31.8 Americium-241 and radium-226 in the form of calibration or reference sources. (a..., americium-241 or radium-226 in the form of calibration or reference sources: (1) Any person in a...

  6. Uncertainty analysis of doses from ingestion of plutonium and americium.

    Science.gov (United States)

    Puncher, M; Harrison, J D

    2012-02-01

    Uncertainty analyses have been performed on the biokinetic model for americium currently used by the International Commission on Radiological Protection (ICRP), and the model for plutonium recently derived by Leggett, considering acute intakes by ingestion by adult members of the public. The analyses calculated distributions of doses per unit intake. Those parameters having the greatest impact on prospective doses were identified by sensitivity analysis; the most important were the fraction absorbed from the alimentary tract, f(1), and rates of uptake from blood to bone surfaces. Probability distributions were selected based on the observed distribution of plutonium and americium in human subjects where possible; the distributions for f(1) reflected uncertainty on the average value of this parameter for non-specified plutonium and americium compounds ingested by adult members of the public. The calculated distributions of effective doses for ingested (239)Pu and (241)Am were well described by log-normal distributions, with doses varying by around a factor of 3 above and below the central values; the distributions contain the current ICRP Publication 67 dose coefficients for ingestion of (239)Pu and (241)Am by adult members of the public. Uncertainty on f(1) values had the greatest impact on doses, particularly effective dose. It is concluded that: (1) more precise data on f(1) values would have a greater effect in reducing uncertainties on doses from ingested (239)Pu and (241)Am, than reducing uncertainty on other model parameter values and (2) the results support the dose coefficients (Sv Bq(-1) intake) derived by ICRP for ingestion of (239)Pu and (241)Am by adult members of the public.

  7. Recovery of americium-241 from aged plutonium metal

    International Nuclear Information System (INIS)

    After separation and purification, both actinides were precipitated as oxalates and calcined. A large-scale process was developed using dissolution, separation, purification, precipitation, and calcination. Efforts were made to control corrosion, to avoid product contamination, to keep the volume of process and waste solutions manageable, and to denitrate solutions with formic acid. The Multipurpose Processing Facility (MPPF), designed for recovery of transplutonium isotopes, was used for the first time for the precipitation and calcination of americium. Also, for the first time,, large-scale formic acid denitration was performed in a canyon vessel at SRP

  8. Effect of 241-americium on bone marrow stroma

    International Nuclear Information System (INIS)

    The regulation of haemopoiesis occurs via complex interactions between the stroma and the haemopoietic cells. An attempt to further clarifying the mechanisms and the exact role of the stroma in the regulation was made in a study. Results revealed that the murine bone marrow stromal cells are highly radiosensitive after injection with 241-americium and can thus be considered as a target population after internal contamination. In addition, observations are made which may be important for risk estimation for the developing animal and during pregnancy. Contamination in utero and by lactation shows persistent damage up to 1 year after contamination at an average annual dose of 5 cGy. (author)

  9. 10 CFR 600.232 - Equipment.

    Science.gov (United States)

    2010-01-01

    ... 10 Energy 4 2010-01-01 2010-01-01 false Equipment. 600.232 Section 600.232 Energy DEPARTMENT OF... Equipment. (a) Title. Subject to the obligations and conditions set forth in this section, title to equipment acquired under a grant or subgrant will vest upon acquisition in the grantee or...

  10. 9 CFR 2.32 - Personnel qualifications.

    Science.gov (United States)

    2010-01-01

    ... least the following areas: (1) Humane methods of animal maintenance and experimentation, including: (i... 9 Animals and Animal Products 1 2010-01-01 2010-01-01 false Personnel qualifications. 2.32 Section 2.32 Animals and Animal Products ANIMAL AND PLANT HEALTH INSPECTION SERVICE, DEPARTMENT...

  11. 27 CFR 31.232 - Wine bottling.

    Science.gov (United States)

    2010-04-01

    .... The decanting of wine by caterers or other retail dealers for table or room service, banquets, and... 27 Alcohol, Tobacco Products and Firearms 1 2010-04-01 2010-04-01 false Wine bottling. 31.232... OF THE TREASURY LIQUORS ALCOHOL BEVERAGE DEALERS Miscellaneous § 31.232 Wine bottling. Each...

  12. 48 CFR 232.7004 - Contract clause.

    Science.gov (United States)

    2010-10-01

    ... OF DEFENSE GENERAL CONTRACTING REQUIREMENTS CONTRACT FINANCING Electronic Submission and Processing of Payment Requests and Receiving Reports 232.7004 Contract clause. Except as provided in 232.7002(a... 48 Federal Acquisition Regulations System 3 2010-10-01 2010-10-01 false Contract clause....

  13. 7 CFR 23.2 - Administration.

    Science.gov (United States)

    2010-01-01

    ... 7 Agriculture 1 2010-01-01 2010-01-01 false Administration. 23.2 Section 23.2 Agriculture Office... Administration. (a) Title V will be administered by the Administrators of the Extension Service and the... Act of 1914 and the Hatch Act (as amended), August 11, 1955, the administration of the programs...

  14. 17 CFR 232.102 - Exhibits.

    Science.gov (United States)

    2010-04-01

    ... pursuant to the schedule's general instructions. See Rule 311(b) of Regulation S-T (17 CFR 232.311(b)). (b... registered investment company or a business development company). (d) Each electronic filing requiring... AND REGULATIONS FOR ELECTRONIC FILINGS Electronic Filing Requirements § 232.102 Exhibits. (a)...

  15. 24 CFR 232.805 - Insurance premiums.

    Science.gov (United States)

    2010-04-01

    ... 24 Housing and Urban Development 2 2010-04-01 2010-04-01 false Insurance premiums. 232.805 Section... FACILITIES Contract Rights and Obligations Premiums § 232.805 Insurance premiums. (a) First premium. The... insurance premium equal to one percent of the original face amount of the note. (b) Second premium....

  16. Preferential decorporation of americium by pulmonary administration of DTPA dry powder after inhalation of aged PuO2 containing americium in rats

    International Nuclear Information System (INIS)

    After inhalation of plutonium oxides containing various percentages of americium in rats, we identified an acellular transient pulmonary compartment, the epithelial lining fluid (ELF), in which a fraction of actinide oxides dissolve prior to absorption and subsequent extrapulmonary deposit. Chelation therapy is usually considered to be poorly efficient after inhalation of actinide oxides. However, in the present study, prompt pulmonary administration of diethylenetriaminepentaacetic acid (DTPA) as a dry powder led to a decrease in actinide content in ELF together with a limitation of bone and liver deposits. Because americium is more soluble than plutonium, higher amounts of americium were found in ELF, extrapulmonary tissues and urine. Our results also demonstrated that the higher efficacy of DTPA on americium compared to plutonium in ELF induced a preferential inhibition of extrapulmonary deposit and a greater urinary excretion of americium compared to plutonium. All together, our data justify the use of an early and local DTPA treatment after inhalation of plutonium oxide aerosols in which americium can be in high proportion such as in aged compounds. (authors)

  17. 49 CFR Appendix B to Part 232 - Part 232 Prior to May 31, 2001 as Clarified Effective April 10, 2002

    Science.gov (United States)

    2010-10-01

    ... Locomotive Inspection and United States Safety Appliance Acts and related orders and regulations of the... percentage. 232.2Drawbars; standard height. 232.3Power brakes and appliances for operating power-brake systems. 232.10General rules; locomotives. 232.11Train air brake system tests. 232.12Initial terminal...

  18. Kilogram-scale purification of americium by ion exchange

    Energy Technology Data Exchange (ETDEWEB)

    Wheelwright, E. J.

    1979-01-01

    Sequential anion and cation exchange processes have been used for the final purification of /sup 241/Am recovered during the reprocessing of aged plutonium metallurgical scrap. Plutonium was removed by absorption of Dowex 1, X-3.5 (30 to 50 mesh) anion exchange resin from 6.5 to 7.5 M HNO/sub 3/ feed solution. Following a water dilution to 0.75 to 1.0 M HNO/sub 3/, americium was absorbed on Dowex 50W, X-8 (50 to 100 mesh) cation exchange resion. Final purification was accomplished by elution of the absorbed band down 3 to 4 successive beds of the same resin, preloaded with Zn/sup 2 +/, with an NH/sub 4/OH buffered chelating agent. The recovery of mixed /sup 241/Am-/sup 243/Am from power reactor reprocessing waste has been demonstrated. Solvent extraction was used to recover a HNO/sub 3/ solution of mixed lanthanides and actinides from waste generated by the reprocessng of 13.5 tons of Shippingport Power Reactor blanket fuel. Sequential cation exchange band-displacement processes were then used to separate americium and curium from the lanthanides and then to separate approx. 60 g of /sup 244/Cm from 1000 g of mixed /sup 241/Am-/sup 243/Am.

  19. Analytical performance of radiochemical method for americium determination in urine

    International Nuclear Information System (INIS)

    This paper presents an analytical method developed and adapted for separation and analysis of Plutonium (Pu) isotopes and Americium (Am) in urine samples. The proposed method will attend the demand of internal exposure monitoring program for workers involved mainly with dismantling rods and radioactive smoke detectors. In this experimental procedure four steps are involved as preparation of samples, sequential radiochemical separation, preparation of the source for electroplating and quantification by alpha spectrometry. In the first stage of radiochemical separation, plutonium is conventionally isolated employing the anion exchange technique. Americium isolation is achieved sequentially by chromatographic extraction (Tru.spec column) from the load and rinse solutions coming from the anion exchange column. The 243Am tracer is added into the sample as chemical yield monitors and to correct the results improving the precision and accuracy. The mean recovery obtained is 60%, and the detection limit for 24h urine sample is 1.0 mBq L-1 in accordance with the literature. Based in the preliminary results, the method is appropriate to be used in monitoring programme of workers with a potential risk of internal contamination. (author)

  20. Development of separation techniques of americium from reprocessing solution

    International Nuclear Information System (INIS)

    Americium(Am) and neptunium(Np) finally transfer to the waste stream in the current PUREX reprocessing process. As an option, some methods have been developed to recover Am and Np from the waste stream to decrease long-term toxicity of the high level waste. The most stable valence state of Am is III, but TBP (tri-n-butyl phosphate) which is an extractant used in the PUREX reprocessing does not extract Am(III). Therefore, some special extractants have been developed to recover Am(III). However, they also extract rare-earth elements(REs), which necessitates the separation process for Am from REs. We have been developing a separation process which consists of valence control of Am to the VI state and its extraction with TBP. This process allows Am recovery from reprocessing solution and Am separation from REs simultaneously. Americium(III) is oxidized to Am(VI) by electrochemical oxidation and chemical oxidation using peroxodisulfate ammonium and silver nitrate. The latter was adopted here because the chemical oxidation reaction proceeds faster than the electrochemical method. Reaction mechanisms of oxidation and extraction were investigated. Based on the mechanisms, we found that extraction efficiency could be improved and waste generation could be minimized. (author)

  1. Selective leaching studies of deep-sea sediments loaded with americium, neptunium and plutonium

    International Nuclear Information System (INIS)

    A series of selective leaching experiments were undertaken to investigate the solid phase speciation and distribution of americium, neptunium and plutonium which had been experimentally loaded onto different marine sediment types. The chemical leaches employed showed rather poor selectivity but certain trends were evident. Adsorption was not by ion exchange. Americium showed a preferential affinity for carbonate and plutonium for organic matter. Neptunium appeared to have no preferential affinities. Americium was sorbed by acetic acid residues (CaCO3 removed) and by unleached carbonate-rich sediments with equal efficiency. This indicates that it is able to diversify its solid phase affinity/distribution depending upon which solid phases are available. (author)

  2. Dicty_cDB: SLB232 [Dicty_cDB

    Lifescience Database Archive (English)

    Full Text Available SL (Link to library) SLB232 (Link to dictyBase) - G22385 DDB0217102 Contig-U16083-1 SLB...232P (Link to Original site) SLB232F 620 SLB232Z 733 SLB232P 1353 - - Show SLB232 Library SL (Link to library) Clone ID SLB...Contig-U16083-1 Original site URL http://dictycdb.biol.tsukuba.ac.jp/CSM/SL/SLB2-B/SLB...232Q.Seq.d/ Representative seq. ID SLB232P (Link to Original site) Representative DNA sequence >SLB232 (SLB232Q) /CSM/SL/SLB...2-B/SLB232Q.Seq.d/ ATATATTTAAAAATAATAAAATAAAAAAAAAAAAAAAAACTGTATTAAAAAAAAAAAAAA TTGTAGT

  3. Pretreatment of americium/curium solutions for vitrification

    International Nuclear Information System (INIS)

    Vitrification will be used to stabilize an americium/curium (Am/Cm) solution presently stored in F-Canyon for eventual transport to the heavy isotope programs at Oak Ridge National Laboratory. Prior to vitrification, an in-tank oxalate precipitation and a series of oxalic/nitric acid washes will be used to separate these elements and lanthanide fission products from the bulk of the uranium and metal impurities present in the solution. Pretreatment development experiments were performed to understand the behavior of the lanthanides and the metal impurities during the oxalate precipitation and properties of the precipitate slurry. The results of these experiments will be used to refine the target glass composition allowing optimization of the primary processing parameters and design of the solution transfer equipment

  4. Plutonium and americium in sediments of Lithuanian lakes

    International Nuclear Information System (INIS)

    The assessment of contribution of the global and the Chernobyl NPP (Nuclear Power Plant) accident plutonium and americium to plutonium pollution in sediments of Lithuanian lakes is presented. Theoretical evaluation of activity ratios of 238Pu/239+240Pu and 241Pu/239+240Pu in the reactor of unit 4 of the Chernobyl NPP before the accident was performed by means of the ORIGEN-ARP code from the SCALE 4.4A program package. Non-uniform distribution of radionuclides in depositions on the Lithuanian territory after nuclear weapon tests and the Chernobyl NPP accident is experimentally observed by measuring the lake sediment pollution with actinides. The activity concentration of sediments polluted with plutonium ranges from 2.0 ± 0.5 Bq/kg d.w. (dry weight) in Lake Asavelis to 14 ± 2 Bq/kg d.w. in Lake Juodis. The ratio of activity concentrations of plutonium isotopes 238Pu/239+240Pu measured by α-spectrometry in the 10-cm-thick upper layer of bottom sediment varies from 0.03 in Lake Juodis to 0.3 in Lake Zuvintas. The analysis of the ratio values shows that the deposition of the Chernobyl origin plutonium is prevailing in southern and south-western regions of Lithuania. Plutonium of nuclear weapon tests origin in sediments of lakes is observed on the whole territory of Lithuania, and it is especially distinct in central Lithuania. The americium activity due to 241Pu decay after the Chernobyl NPP accident and global depositions in bottom sediments of Lithuanian lakes has been evaluated to be from 0.9 to 5.7 Bq/kg. (author)

  5. Kinetic parameters of transformation of americium and plutonium physicochemical forms in podsol soils

    International Nuclear Information System (INIS)

    Kinetic parameters of transformation of americium and plutonium physicochemical forms have been estimated and the prognosis of fixing and remobilization of these nuclides in podsol soils have been made on that basis in the work. (authors)

  6. Calibration procedures for in vivo sodium iodide spectrometry of plutonium and americium in the human lung

    International Nuclear Information System (INIS)

    This paper describes the calibration techniques and associated error analysis for the in vivo measurement by NaI spectrometry of heavy elements in the lung, specifically plutonium and americium. A very brief description of the instrumentation system is included

  7. Relativistic density functional theory modeling of plutonium and americium higher oxide molecules

    Science.gov (United States)

    Zaitsevskii, Andréi; Mosyagin, Nikolai S.; Titov, Anatoly V.; Kiselev, Yuri M.

    2013-07-01

    The results of electronic structure modeling of plutonium and americium higher oxide molecules (actinide oxidation states VI through VIII) by two-component relativistic density functional theory are presented. Ground-state equilibrium molecular structures, main features of charge distributions, and energetics of AnO3, AnO4, An2On (An=Pu, Am), and PuAmOn, n = 6-8, are determined. In all cases, molecular geometries of americium and mixed plutonium-americium oxides are similar to those of the corresponding plutonium compounds, though chemical bonding in americium oxides is markedly weaker. Relatively high stability of the mixed heptoxide PuAmO7 is noticed; the Pu(VIII) and especially Am(VIII) oxides are expected to be unstable.

  8. 48 CFR 232.1110 - Solicitation provision and contract clauses.

    Science.gov (United States)

    2010-10-01

    ... contract clauses. 232.1110 Section 232.1110 Federal Acquisition Regulations System DEFENSE ACQUISITION REGULATIONS SYSTEM, DEPARTMENT OF DEFENSE GENERAL CONTRACTING REQUIREMENTS CONTRACT FINANCING Electronic Funds Transfer 232.1110 Solicitation provision and contract clauses. Use the clause at 252.232-7009,...

  9. Distribution of uranium, americium and plutonium in the biomass of freshwater macrophytes

    Energy Technology Data Exchange (ETDEWEB)

    Zotina, T.A.; Kalacheva, G.S.; Bolsunovsky, A.YA. [Institute of Biophysics SB RAS, Akademgorodok, Krasnoyarsk (Russian Federation)

    2010-07-01

    Accumulation of uranium ({sup 238}U), americium ({sup 241}Am) and plutonium ({sup 242}Pu) and their distribution in cell compartments and biochemical components of the biomass of aquatic plants Elodea canadensis, Ceratophyllum demersum, Myrioplyllum spicatum and aquatic moss Fontinalis antipyretica have been investigated in laboratory batch experiments. Isotopes of uranium, americium and plutonium taken up from the water by Elodea canadensis apical shoots were mainly absorbed by cell walls, plasmalemma and organelles. A small portion of isotopes (about 6-13 %) could be dissolved in cytoplasm. The major portion (76-92 %) of americium was bound to cell wall cellulose-like polysaccharides of Elodea canadensis, Myriophyllum spicatum, Ceratophyllum demersum and Fontinalis antipyretica, 8-23 % of americium activity was registered in the fraction of proteins and carbohydrates, and just a small portion (< 1%) in lipid fraction. The distribution of plutonium in the biomass fraction of Elodea was similar to that of americium. Hence, americium and plutonium had the highest affinity to cellulose-like polysaccharides in Elodea biomass. Distribution of uranium in the biomass of Elodea differed essentially from that of transuranium elements: a considerable portion of uranium was recorded in the fraction of protein and carbohydrates (51 %). From our data we can assume that uranium has higher affinity to carbohydrates than proteins. (authors)

  10. Dicty_cDB: SLE232 [Dicty_cDB

    Lifescience Database Archive (English)

    Full Text Available SL (Link to library) SLE232 (Link to dictyBase) - - - Contig-U16255-1 SLE232F (Link... to Original site) SLE232F 614 - - - - - - Show SLE232 Library SL (Link to library) Clone ID SLE232 (Link to dict...yBase) Atlas ID - NBRP ID - dictyBase ID - Link to Contig Contig-U16255-1 Original site URL http://dict...PSSGFTDFIPSNATCSSLNCNAQQMSCKYVQQACHETSCCPDIPQC QIPATGGGPATGSATGQGTSGGTPGSCDKVNCPNGYICTIVNQLAVCVSPSSSSSSSSST ...CHETSCCPDIPQC QIPATGGGPATGSATGQGTSGGTPGSCDKVNCPNGYICTIVNQLAVCVSPSSSSSSSSST TGSHTTTGGSTTGSHTTTGGSTTGSHTTTGGSA

  11. Effect of americium-241 on luminous bacteria. Role of peroxides

    Energy Technology Data Exchange (ETDEWEB)

    Alexandrova, M., E-mail: maka-alexandrova@rambler.r [Siberian Federal University, Svobodny 79, 660041 Krasnoyarsk (Russian Federation); Rozhko, T. [Siberian Federal University, Svobodny 79, 660041 Krasnoyarsk (Russian Federation); Vydryakova, G. [Institute of Biophysics SB RAS, Akademgorodok 50, 660036 Krasnoyarsk (Russian Federation); Kudryasheva, N. [Siberian Federal University, Svobodny 79, 660041 Krasnoyarsk (Russian Federation); Institute of Biophysics SB RAS, Akademgorodok 50, 660036 Krasnoyarsk (Russian Federation)

    2011-04-15

    The effect of americium-241 ({sup 241}Am), an alpha-emitting radionuclide of high specific activity, on luminous bacteria Photobacterium phosphoreum was studied. Traces of {sup 241}Am in nutrient media (0.16-6.67 kBq/L) suppressed the growth of bacteria, but enhanced luminescence intensity and quantum yield at room temperature. Lower temperature (4 {sup o}C) increased the time of bacterial luminescence and revealed a stage of bioluminescence inhibition after 150 h of bioluminescence registration start. The role of conditions of exposure the bacterial cells to the {sup 241}Am is discussed. The effect of {sup 241}Am on luminous bacteria was attributed to peroxide compounds generated in water solutions as secondary products of radioactive decay. Increase of peroxide concentration in {sup 241}Am solutions was demonstrated; and the similarity of {sup 241}Am and hydrogen peroxide effects on bacterial luminescence was revealed. The study provides a scientific basis for elaboration of bioluminescence-based assay to monitor radiotoxicity of alpha-emitting radionuclides in aquatic solutions. - Highlights: {yields} Am-241 in water solutions (A = 0.16-6.7 kBq/L) suppresses bacterial growth.{yields} Am-241 (A = 0.16-6.7 kBq/L) stimulate bacterial luminescence. {yields} Peroxides, secondary radiolysis products, cause increase of bacterial luminescence.

  12. 48 CFR 232.070 - Responsibilities.

    Science.gov (United States)

    2010-10-01

    ... DoD contract financing, including DoD contract financing policies and important related procedures... operations. Refer specific cases involving financing policy or important procedural issues to OUSD(AT&L)DPAP... OF DEFENSE GENERAL CONTRACTING REQUIREMENTS CONTRACT FINANCING 232.070 Responsibilities. (a)...

  13. 42 CFR 23.2 - Definitions.

    Science.gov (United States)

    2010-10-01

    ... regulation (42 CFR part 5). National Health Service Corps site means the entity to which personnel have been... HEALTH SERVICE, DEPARTMENT OF HEALTH AND HUMAN SERVICES PERSONNEL NATIONAL HEALTH SERVICE CORPS Assignment of National Health Service Corps Personnel § 23.2 Definitions. As used in this......

  14. 24 CFR 232.885 - Insurance benefits.

    Science.gov (United States)

    2010-04-01

    ... 24 Housing and Urban Development 2 2010-04-01 2010-04-01 false Insurance benefits. 232.885 Section... DEVELOPMENT MORTGAGE AND LOAN INSURANCE PROGRAMS UNDER NATIONAL HOUSING ACT AND OTHER AUTHORITIES MORTGAGE INSURANCE FOR NURSING HOMES, INTERMEDIATE CARE FACILITIES, BOARD AND CARE HOMES, AND ASSISTED...

  15. 48 CFR 52.232-17 - Interest.

    Science.gov (United States)

    2010-10-01

    ... 48 Federal Acquisition Regulations System 2 2010-10-01 2010-10-01 false Interest. 52.232-17... Interest. As prescribed in 32.611(a) and (b), insert the following clause: INTEREST (OCT 2010) (a) Except... Contractor to the Government under this contract shall bear simple interest from the date due until...

  16. 43 CFR 17.232 - Postsecondary education.

    Science.gov (United States)

    2010-10-01

    ... promulgated by the Department of Education at 34 CFR part 104, subpart E. ... 43 Public Lands: Interior 1 2010-10-01 2010-10-01 false Postsecondary education. 17.232 Section 17... Postsecondary education. This section applies to postsecondary education and activities, including...

  17. 10 CFR 32.57 - Calibration or reference sources containing americium-241 or radium-226: Requirements for license...

    Science.gov (United States)

    2010-01-01

    ... or radium-226: Requirements for license to manufacture or initially transfer. 32.57 Section 32.57... americium-241 or radium-226: Requirements for license to manufacture or initially transfer. An application... containing americium-241 or radium-226, for distribution to persons generally licensed under § 31.8 of...

  18. Separation and determination of americium in low-level alkaline waste of NPP origin

    Science.gov (United States)

    Todorov, B.; Djingova, R.; Nikiforova, A.

    2006-01-01

    The aim of this work is to develop a short and cost-saving procedure for the determination of 241Am in sludge sample of the alkaline low-level radioactive waste (LL LRAW) collected from Nuclear Power Plant “Kozloduy”. The determination of americium was a part of a complex analytical approach, where group actinide separation was achieved. An anion exchange was used for separation of americium from uranium, plutonium and iron. For the separation of americium extraction with diethylhexyl phosphoric acid (DEHPA) was studied. The final radioactive samples were prepared by micro co-precipitation with NdF3, counted by alpha and gamma spectrometry. The procedure takes 2 hours. The recovery yield of the procedure amounts to (95 ± 1.5)% and the detection limit is 53 mBq/kg 241Am (t=150 000 s). The analytical procedure was applied for actual liquid wastes and results were compared to standard procedure.

  19. 46 CFR 232.4 - Balance sheet accounts.

    Science.gov (United States)

    2010-10-01

    ... Administration's Dividend Policy for Operators Receiving ODS (46 CFR part 283), accounting information for... 46 Shipping 8 2010-10-01 2010-10-01 false Balance sheet accounts. 232.4 Section 232.4 Shipping... ACTIVITIES UNIFORM FINANCIAL REPORTING REQUIREMENTS Balance Sheet § 232.4 Balance sheet accounts....

  20. 49 CFR 232.613 - End-of-train devices.

    Science.gov (United States)

    2010-10-01

    ... 49 Transportation 4 2010-10-01 2010-10-01 false End-of-train devices. 232.613 Section 232.613... EQUIPMENT; END-OF-TRAIN DEVICES Electronically Controlled Pneumatic (ECP) Braking Systems § 232.613 End-of-train devices. (a) An ECP-EOT device shall, at a minimum, serve as the final node on the ECP...

  1. Isotopic and elemental composition of plutonium/americium oxides influence pulmonary and extra-pulmonary distribution after inhalation in rats

    International Nuclear Information System (INIS)

    The biodistribution of plutonium and americium has been studied in a rat model after inhalation of two PuO2 powders in lungs and extra-pulmonary organs from 3 d to 3 mo. The main difference between the two powders was the content of americium (approximately 46% and 4.5% of total alpha activity). The PuO2 with a higher proportion of americium shows an accelerated transfer of activity from lungs to blood as compared to PuO2 with the lower americium content, illustrated by increased urinary excretion and higher bone and liver actinide retention. The total alpha activity measured reflects mostly the americium biological behavior. The activity contained in epithelial lining fluid, recovered in the acellular phase of broncho-alveolar lavages, mainly contains americium, whereas plutonium remains trapped in macrophages. Epithelial lining fluid could represent a transitional pulmonary compartment prior to translocation of actinides to the blood and subsequent deposition in extra-pulmonary retention organs. In addition, differential behaviors of plutonium and americium are also observed between the PuO2 powders with a higher dissolution rate for both plutonium and americium being obtained for the PuO2 with the highest americium content. Our results indicate that the biological behavior of plutonium and americium after translocation into blood differ two-fold: (1) for the two actinides for the same PuO2 aerosol, and (2) for the same actinide from the two different aerosols. These results highlight the importance of considering the specific behavior of each contaminant after accidental pulmonary intake when assessing extra-pulmonary deposits from the level of activity excreted in urine or for therapeutic strategy decisions. (authors)

  2. Isotopic and elemental composition of plutonium/americium oxides influence pulmonary and extra-pulmonary distribution after inhalation in rats.

    Science.gov (United States)

    Van der Meeren, A; Grémy, O

    2010-09-01

    The biodistribution of plutonium and americium has been studied in a rat model after inhalation of two PuO(2) powders in lungs and extra-pulmonary organs from 3 d to 3 mo. The main difference between the two powders was the content of americium (approximately 46% and 4.5% of total alpha activity). The PuO(2) with a higher proportion of americium shows an accelerated transfer of activity from lungs to blood as compared to PuO(2) with the lower americium content, illustrated by increased urinary excretion and higher bone and liver actinide retention. The total alpha activity measured reflects mostly the americium biological behavior. The activity contained in epithelial lining fluid, recovered in the acellular phase of broncho-alveolar lavages, mainly contains americium, whereas plutonium remains trapped in macrophages. Epithelial lining fluid could represent a transitional pulmonary compartment prior to translocation of actinides to the blood and subsequent deposition in extra-pulmonary retention organs. In addition, differential behaviors of plutonium and americium are also observed between the PuO(2) powders with a higher dissolution rate for both plutonium and americium being obtained for the PuO(2) with the highest americium content. Our results indicate that the biological behavior of plutonium and americium after translocation into blood differ two-fold: (1) for the two actinides for the same PuO(2) aerosol, and (2) for the same actinide from the two different aerosols. These results highlight the importance of considering the specific behavior of each contaminant after accidental pulmonary intake when assessing extra-pulmonary deposits from the level of activity excreted in urine or for therapeutic strategy decisions.

  3. Adsorption-desorption characteristics of plutonium and americium with sediment particles in the estuarine environment: studies using plutonium-237 and americium-241

    International Nuclear Information System (INIS)

    The particle formation of plutonium and americium, their adsorption onto fresh water sediments and the desorption from the sediments in sea water were studied in the Laboratory under simulated river-estuary conditions, using γ-emitting plutonium-237 and americium-241. The results of the experiments show that the particle formation of plutonium depends on its valence states, on pH and on the salinity of the medium. For river water at pH4, some 25%, 20% and 30% of the added 237Pu was in particulate form, larger than 0.45 μm, for Pu (III), Pu (IV) and Pu (VI), respectively, while 65%, 90% and 50% of the respective valence states was associated with particles at pH 8. In sea water the general pattern remains similar, although Pu (VI) is more soluble in sea water owing to higher ligand concentrations for carbonate and bicarbonate complexes. The pH-dependency of particle formation of Am (III) is more steep than that of plutonium and seems to be influenced by colloidal substances occurring in the experimental media. The adsorption-desorption characteristics of plutonium and americium with the sediment in river water as well as sea water reflect the characteristics of their particle formation, being dependent upon such properties as valence states, the pH and salinity of the medium. A sewage effluent added to the media has small but measurable effects on the adsorption-desorption processes of plutonium. (author)

  4. Cesium-137 and americium-241 distribution by granulometric fractions of soil at Azgir test site grounds

    International Nuclear Information System (INIS)

    In measurements of radionuclide specific content in surface soil layer of contaminated territories it is important to determine in what agglomerations of soil particles there is the highest radionuclide concentration. For this purpose granulometric composition of soil at Azgir test site was studied and cesium-137 and americium-241 distribution by soil fractions was researched. (author)

  5. Apparatus for fabrication of americium- beryllium neutron sources prevents capsule contamination

    Science.gov (United States)

    Mohr, W. C.; Van Loom, J. A.

    1967-01-01

    Modified gloved enclosure is used to fill a capsule with a mixture of americium and beryllium radioactive powders to seal weld the opening, and to test it for leaks. It contains a horizontal partition, vortex mixer, mounting press, welder, test vessel, and radiation shielding to prevent surface contamination.

  6. Evaluation of the readsorption of plutonium and americium in dynamic fractionations of environmental solid samples

    DEFF Research Database (Denmark)

    Petersen, Roongrat; Hou, Xiaolin; Hansen, Elo Harald

    2008-01-01

    extractions. The degree of readsorption in dynamic and conventional batch extraction systems are compared and evaluated by using a double-spiking technique. A high degree of readsorption of plutonium and americium (>75%) was observed in both systems, and they also exhibited similar distribution patterns...

  7. Effect of bone-status on retention and distribution of americium-241 in bones of small rodents

    International Nuclear Information System (INIS)

    Forced physical exercise before and after application of americium-241 resulted in only small changes in bone-structure and behaviour of the radionuclide in bone. Feeding of a low phosphorus or low calcium diet resulted in an increased excretion of americium from bone, whereby Zn-DTPA as chelating agent removed an additional fraction of the radionuclide from bone. Low calcium diet and simultaneous continuous infusion of pharmacological doses of vitamin D-hormones didn't increase the excretion of americium more than the low calcium diet alone. (orig.)

  8. Interaction and diffusion transport of americium in soils

    Energy Technology Data Exchange (ETDEWEB)

    Ramirez-Guinart, Oriol; Rigol, Anna; Vidal, Miquel [Analytical Chemistry department, Faculty of Chemistry, University of Barcelona, Marti i Franques 1-11, 08028, Barcelona (Spain)

    2014-07-01

    The final disposal of High Level Radioactive Wastes (HLRW) is based on its long-term storage in underground facilities located in geological stable sites with a multi-barrier system, the so called Deep Geological Repositories (DGR), that will keep HLRW confined for >10.000 years. After this period of time, leachates rich in long-live radioisotopes might escape from DGR and start to transport towards the biosphere. There is still a lack of information concerning the interaction and transport in soils of some radionuclides present in HLRW, especially for radionuclides that present a high sorption, such as americium (Am). Having reliable information about the mobility of radionuclides in soils is crucial in order to develop risk assessment models and to take proper decisions in case of soil contamination. The aim of the present work was, by means of laboratory scale experiments, to study the interaction and, for first time, to evaluate the diffusion transport of {sup 241}Am in soils. The {sup 241}Am interaction in soils was assessed by applying sorption batch assays to 20 soil samples with contrasted edaphic properties which allowed us to quantify the solid-liquid distribution coefficient (K{sub d}) and desorption percentage. K{sub d} (Am) values ranged from 10{sup 3} to 10{sup 5} L kg{sup -1} and desorption percentages were always less than 2% which denoted a high capacity of the soil to incorporate the Am and a low reversibility of the sorption process. The influence of soil properties in {sup 241}Am interaction was studied by means of multiple linear and multivariate regressions. Although a single correlation between K{sub d} (Am) values and a soil property was not found, the main properties affecting {sup 241}Am interaction in soils were soil pH, carbonate and organic matter contents in the soil. Finally, additional batch assays at different controlled pH were done to study Am sorption as a function of the contact solution pH. A variation of the Am sorption

  9. SKIN DOSIMETRY IN CONDITIONS OF ITS CONSTANT SURFACE CONTAMINATION WITH SOLUTIONS OF PLUTONIUM-239 AND AMERICIUM-241

    Directory of Open Access Journals (Sweden)

    E. B. Ershov

    2012-01-01

    Full Text Available The article considers, on the basis of experimental data, the issue of assessing dose burdens to the skin basal layer in conditions of its permanent contamination with solutions of plutonium-239 and americium-241 and subsequent decontamination.

  10. Influence of biofilms on migration of uranium, americium and europium in the environment; Einfluss von Biofilmen auf das Migrationsverhalten von Uran, Americium und Europium in der Umwelt

    Energy Technology Data Exchange (ETDEWEB)

    Baumann, Nils; Zirnstein, Isabel; Arnold, Thuro

    2015-07-01

    The report on the influence of biofilms on migration of uranium, americium and europium in the environment deals with the contamination problems of uranium mines such as SDAG WISMUT in Saxonia and Thuringia. In mine waters microorganisms form a complex microbiological biocoenosis in spite of low pH values and high heavy metal concentrations including high uranium concentrations. The analyses used microbiological methods like confocal laser scanning microscopy and molecular-biological techniques. The interactions of microorganism with fluorescent radioactive heavy metal ions were performed with TRLFS (time resolved laser-induced fluorescence spectroscopy).

  11. Liquid-liquid extraction separation and sequential determination of plutonium and americium in environmental samples by alpha-spectrometry

    International Nuclear Information System (INIS)

    A procedure is described by which plutonium and americium can be determined in environmental samples. The sample is leached with nitric acid and hydrogen peroxide, and the two elements are co-precipitated with ferric hydroxide and calcium oxalate. The calcium oxalate is incinerated at 4500 and the ash is dissolved in nitric acid. Plutonium is extracted with tri-n-octylamine solution in xylene from 4M nitric acid and stripped with ammonium iodide/hydrochloric acid. Americium is extracted with thenoyltrifluoroacetone solution in xylene at pH 4 together with rare-earth elements and stripped with 1M nitric acid. Americium and the rare-earth elements thus separated are sorbed on Dowex 1 x 4 resin from 1M nitric acid in 93% methanol, the rare-earth elements are eluted with 0.1M hydrochloric acid/0.5M ammonium thiocyanate/80% methanol and the americium is finally eluted with 1.5M hydrochloric acid in 86% methanol. Plutonium and americium in each fraction are electro-deposited and determined by alpha-spectrometry. Overall average recoveries are 81% for plutonium and 59% for americium. (author)

  12. Influence of environmental factors on the gastrointestinal absorption of plutonium and americium

    International Nuclear Information System (INIS)

    The absorption of plutonium and americium from the gastrointestinal tract was studied, using adult hamsters and rabbits. Both actinides were administered as inorganic compounds, as organic complexes with naturally occurring chelating agents, and in a biologically incorporated form in liver tissues. The absorption of the tetravalent and hexavalent forms of plutonium were compared and the effect of protracted administration at very low concentrations was investigated. In addition, plutonium uptake from contaminated sediments and grass, collected near a nuclear-fuel reprocessing plant, was measured. The results of these studies suggest that chronic exposure of man to plutonium and americium in food and water will not lead to any substantial increase in their gastrointestinal absorption above the values currently recommended by the International Commission on Radiological Protection to define the occupational exposure of workers

  13. Electrodeposition of americium on a liquid cadmium cathode from a molten salt bath

    International Nuclear Information System (INIS)

    A high-activity experiment involving the electrode position of americium on a liquid cadmium cathode from a LiCl-KCl eutectic with about 3 g of AmO2 was conducted in a shielded cell in the ATALANTE complex. After describing the electrolyzer and the experimental conditions, the authors discuss the preparation of the LiCl-KCl-AmCl3 solution and briefly review its electrochemical properties. It was clearly confirmed that Am(III) reduction on an inert solid cathode occurs in two steps forming Am(II) before Am(0), whereas only one reduction step was observed on liquid cadmium. The main results of this study concern americium electrode position on the liquid cadmium cathode (recovery yields, current densities, problems encountered). The solvent properties of cadmium for actinide/lanthanide separation are discussed. (authors)

  14. Analysis of americium-beryllium neutron source composition using the FRAM code

    Energy Technology Data Exchange (ETDEWEB)

    Hypes, P. A. (Philip A.); Bracken, D. S. (David S.); Sampson, Thomas E.; Taylor, W. A. (Wayne A.)

    2002-01-01

    The FRAM code was originally developed to analyze high-resolution gamma spectra from plutonium items. Its capabilities have since been expanded to include analysis of uranium spectra. The flexibility of the software also enables a capable spectroscopist to use FRAM to analyze spectra in which neither plutonium nor uranium is present in significant amounts. This paper documents the use of FRAM to determine the {sup 239}Pu/{sup 241}Am, {sup 243}Am/{sup 241}Am, {sup 237}Np/{sup 241}Am, and {sup 239}Np/{sup 241}Am ratios in americium-beryllium neutron sources. The effective specific power of each neutron source was calculated from the ratios determined by FRAM in order to determine the americium mass of each of these neutron sources using calorimetric assay. We will also discuss the use of FRAM for the general case of isotopic analysis of nonplutonium, nonuranium items.

  15. Experimental Insight into the Radiation Resistance of Zirconia-Based Americium Ceramics

    International Nuclear Information System (INIS)

    Our works shows that the americium pyrochlore 241Am2Zr2O7 undergoes a phase transition to a defect-fluorite structure along with an unusual volume contraction when subjected to internal radiation from α-emitting actinides. Disorder relaxation proceeds through the simultaneous formation of cation anti sites and oxygen Frenkel pairs. X-ray absorption spectroscopy at the Am-LII and the Zr-K edges reveals that Am-O polyhedra show an increasing disorder with increasing exposure. In contrast, the Zr-O polyhedral units remain highly ordered, while rotating along edges and corners, thereby reducing the structural strain imposed by the growing disorder around americium. We believe it is this particular property of the compound that provides the remarkable resistance to radiation (≥9.4 * 1018) α-decay events g-1 or 0.80 dpa). (authors)

  16. Standard test method for quantitative determination of americium 241 in plutonium by Gamma-Ray spectrometry

    CERN Document Server

    American Society for Testing and Materials. Philadelphia

    1994-01-01

    1.1 This test method covers the quantitative determination of americium 241 by gamma-ray spectrometry in plutonium nitrate solution samples that do not contain significant amounts of radioactive fission products or other high specific activity gamma-ray emitters. 1.2 This test method can be used to determine the americium 241 in samples of plutonium metal, oxide and other solid forms, when the solid is appropriately sampled and dissolved. 1.3 This standard does not purport to address all of the safety concerns, if any, associated with its use. It is the responsibility of the user of this standard to establish appropriate safety and health practices and determine the applicability of regulatory limitations prior to use.

  17. Calcium and zinc DTPA administration for internal contamination with plutonium-238 and americium-241.

    Science.gov (United States)

    Kazzi, Ziad N; Heyl, Alexander; Ruprecht, Johann

    2012-08-01

    The accidental or intentional release of plutonium or americium can cause acute and long term adverse health effects if they enter the human body by ingestion, inhalation, or injection. These effects can be prevented by rapid removal of these radionuclides by chelators such as calcium or zinc diethylenetriaminepentaacetate (calcium or zinc DTPA). These compounds have been shown to be efficacious in enhancing the elimination of members of the actinide family particularly plutonium and americium when administered intravenously or by nebulizer. The efficacy and adverse effects profile depend on several factors that include the route of internalization of the actinide, the type, and route time of administration of the chelator, and whether the calcium or zinc salt of DTPA is used. Current and future research efforts should be directed at overcoming limitations associated with the use of these complex drugs by using innovative methods that can enhance their structural and therapeutic properties.

  18. Final Radiological Assessment of External Exposure for CLEAR-Line Americium Recovery Operations

    Energy Technology Data Exchange (ETDEWEB)

    Davis, Adam C. [Los Alamos National Lab. (LANL), Los Alamos, NM (United States); Belooussova, Olga N. [Los Alamos National Lab. (LANL), Los Alamos, NM (United States); Hetrick, Lucas Duane [Los Alamos National Lab. (LANL), Los Alamos, NM (United States)

    2014-11-12

    Los Alamos National Laboratory is currently planning to implement an americium recovery program. The americium, ordinarily isotopically pure 241Am, would be extracted from existing Pu materials, converted to an oxide and shipped to support fabrication of americium oxide-beryllium neutron sources. These operations would occur in the currently proposed Chloride Extraction and Actinide Recovery (CLEAR) line of glove boxes. This glove box line would be collocated with the currently-operational Experimental Chloride Extraction Line (EXCEL). The focus of this document is to provide an in-depth assessment of the currently planned radiation protection measures and to determine whether or not further design work is required to satisfy design-goal and ALARA requirements. Further, this document presents a history of americium recovery operations in the Department of Energy and high-level descriptions of the CLEAR line operations to provide a basis of comparison. Under the working assumptions adopted by this study, it was found that the evaluated design appears to mitigate doses to a level that satisfies the ALARA-in-design requirements of 10 CFR 835 as implemented by the Los Alamos National Laboratory procedure P121. The analyses indicate that extremity doses would also meet design requirements. Dose-rate calculations were performed using the radiation transport code MCNP5 and doses were estimated using a time-motion study developed in consort with the subject matter expert. A copy of this report and all supporting documentation are located on the Radiological Engineering server at Y:\\Rad Engineering\\2013 PROJECTS\\TA-55 Clear Line.

  19. 48 CFR 232.470 - Advance payment pool.

    Science.gov (United States)

    2010-10-01

    ... 48 Federal Acquisition Regulations System 3 2010-10-01 2010-10-01 false Advance payment pool. 232... Items 232.470 Advance payment pool. (a) An advance payment pool agreement— (1) Is a means of financing... addition to any other advance payment pool agreement at a single contractor location when it is...

  20. 48 CFR 252.232-7000 - Advance payment pool.

    Science.gov (United States)

    2010-10-01

    ... 48 Federal Acquisition Regulations System 3 2010-10-01 2010-10-01 false Advance payment pool. 252... Provisions And Clauses 252.232-7000 Advance payment pool. As prescribed in 232.412-70(a), use the following clause: Advance Payment Pool (DEC 1991) (a) Notwithstanding any other provision of this contract,...

  1. 48 CFR 1852.232-81 - Contract funding.

    Science.gov (United States)

    2010-10-01

    ... 48 Federal Acquisition Regulations System 6 2010-10-01 2010-10-01 true Contract funding. 1852.232... 1852.232-81 Contract funding. As prescribed in 1832.705-270(b), insert the following clause: Contract Funding (JUN 1990) (a) For purposes of payment of cost, exclusive of fee, in accordance with...

  2. 48 CFR 232.501-3 - Contract price.

    Science.gov (United States)

    2010-10-01

    ... 48 Federal Acquisition Regulations System 3 2010-10-01 2010-10-01 false Contract price. 232.501-3 Section 232.501-3 Federal Acquisition Regulations System DEFENSE ACQUISITION REGULATIONS SYSTEM... liquidation rate, or the loss-ratio adjusted rate); or (ii) 100 percent of the funds obligated....

  3. 40 CFR 60.232 - Standard for fluorides.

    Science.gov (United States)

    2010-07-01

    ... 40 Protection of Environment 6 2010-07-01 2010-07-01 false Standard for fluorides. 60.232 Section... Industry: Triple Superphosphate Plants § 60.232 Standard for fluorides. On and after the date on which the... gases which contain total fluorides in excess of 100 g/megagram (Mg) of equivalent P2O5 feed (0.20...

  4. 32 CFR 232.6 - Mandatory loan disclosures.

    Science.gov (United States)

    2010-07-01

    ... 32 National Defense 2 2010-07-01 2010-07-01 false Mandatory loan disclosures. 232.6 Section 232.6... Mandatory loan disclosures. (a) Required information. With respect to any extension of consumer credit (including any consumer credit originated or extended through the internet) to a covered borrower, a...

  5. 24 CFR 232.550 - Accumulation of next premium.

    Science.gov (United States)

    2010-04-01

    ... 24 Housing and Urban Development 2 2010-04-01 2010-04-01 false Accumulation of next premium. 232... of Fire Safety Equipment Eligible Security Instruments § 232.550 Accumulation of next premium. The... date the next annual insurance premium payable by the lender to the Commissioner....

  6. Bidentate organophosphorus extraction of americium and plutonium from Hanford Plutonium Reclamation Facility waste

    Energy Technology Data Exchange (ETDEWEB)

    Schulz, W.W.

    1974-09-01

    Applicability of bidentate organiphosphorus reagents to recovery of americium and plutonium from Hanford's Plutonium Reclamation Facility acid (approx. 2M HNO/sub 3/) waste stream (CAW solution) was studied. A solvent extraction process which employs a 30% DHDECMP (dihexyl-N, N-diethylcarbamylmethylene phosphonate)-CCl/sub 4/ extractant was devised and successfully tested in mixer-settler runs with actual CAW solution. Substitution of DHDECMP for DBBP eliminates the need to perform careful neutralization of unbuffered CAW soluton and increases overall americium recovery from the present 60 to 80% level to greater than or equal to 90%. Disadvantages to such substitution include the high cost (approx. $50/liter) of DHDECMP and the need to purify it (by acid (6M HCl) hydrolysis and alkaline washing) from small amounts of an unidentified impurity which prevents stripping of americium with dilute HNO/sub 3/. Distribution data obtained in this study confirm Siddall's earlier contention that bidentate organophosphorus regents can be used to remove actinides from concentrated high-level Purex process acid waste; a conceptual flowsheet for such an extraction process is given.

  7. Nuclear data evaluation for Th-232

    International Nuclear Information System (INIS)

    In this report the methods, the analysis, and the results of the main neutron nuclear data regarding 232Th are presented, and an evaluated file in ENDF/B-IV format covering the energy range between 10-5eV and 20 MeV is supplied. This file contains evaluated data for total, elastic, inelastic, radiative capture, fission, (n,2n) and (n,3n) cross sections. In addition, the elastic angular distributions, as Legendre coefficients, the average cosine of the scattering angle (laboratory system) (anti μsub(L)), and the average logarithmic energy decrement (xi) for elastic scattering, the prompt, delayed and total average numbers of neutrons per fission, as well as the decay data and the fission yields are included. The data are presented in appropriate forms accepted by the format, namely point-wise or parametric representation. Breit-Wigner Single Level formalism for resonance treatment, optical and coupled channel models for elastic processes and double humped fission model as well as evaporation model have been also used in the data analysis. The largest part of the data are based on experimental measurements, except (n,3n) cross section. The final evaluated data set was checked against format correctness and physical consistency. (author)

  8. 48 CFR 232.072-3 - Cash flow forecasts.

    Science.gov (United States)

    2010-10-01

    ..., DEPARTMENT OF DEFENSE GENERAL CONTRACTING REQUIREMENTS CONTRACT FINANCING 232.072-3 Cash flow forecasts. (a... reliable than the assumptions on which they are based. Most important of these assumptions are—...

  9. Americium(3) coordination chemistry: An unexplored diversity of structure and bonding

    Energy Technology Data Exchange (ETDEWEB)

    Fedosseev, A.M.; Grigoriev, M.S.; Budantseva, N.A. [A.N. Frumkin Institute of Physical Chemistry and Electrochemistry, Moscow (Russian Federation); Guillaumont, D.; Den Auwer, Ch.; Moisy, Ph. [CEA Marcoule, Nuclear Energy Division, RadioChemistry and Processes Department, 30 (France); Le Naour, C.; Simoni, E. [CNRS, University Paris-11 Orsay, IPN, 91 - Orsay (France)

    2010-06-15

    The comparison of the physicochemical behavior of the actinides with that of the lanthanides can be justified by the analogy of their electronic structure, as each of the series is made up of elements corresponding to the filling of a given (n)f atomic shell. However relatively few points of comparison are available, given the lack of available structure for trans-plutonium(III) elements and the additional difficulty of stabilizing coordination complexes of uranium(III) to plutonium(III). This contribution is a focal point of trans-plutonium(III) chemistry and, more specifically, of some americium compounds that have been recently synthesized, all related with hard acid oxygen donor ligands that may be involved in the reprocessing chain of nuclear fuel. After a brief review of the solid hydrates and aquo species for the lanthanide and actinide families, we discuss two types of ligands that have in common three carboxylic groups, namely the amino-tri-acetic acid and the citric acid anions. The additional roles of the nitrogen atom for the first one and of the hydroxy function for the second one are discussed. Accordingly, five new complexes with either americium or lanthanides elements are described: [Co(NH{sub 3}){sub 6}][M(NTA){sub 2}(H{sub 2}O)].8H{sub 2}O with M Nd, Yb and Am, and [Co(NH{sub 3}){sub 6}]{sub 2}K[M{sub 3}(Cit){sub 4}(H{sub 2}O){sub 3}].18H{sub 2}O with Nd and Am cations. In all cases the americium complexes are isostructural with their lanthanide equivalents. (authors)

  10. Americium(3) coordination chemistry: An unexplored diversity of structure and bonding

    International Nuclear Information System (INIS)

    The comparison of the physicochemical behavior of the actinides with that of the lanthanides can be justified by the analogy of their electronic structure, as each of the series is made up of elements corresponding to the filling of a given (n)f atomic shell. However relatively few points of comparison are available, given the lack of available structure for trans-plutonium(III) elements and the additional difficulty of stabilizing coordination complexes of uranium(III) to plutonium(III). This contribution is a focal point of trans-plutonium(III) chemistry and, more specifically, of some americium compounds that have been recently synthesized, all related with hard acid oxygen donor ligands that may be involved in the reprocessing chain of nuclear fuel. After a brief review of the solid hydrates and aquo species for the lanthanide and actinide families, we discuss two types of ligands that have in common three carboxylic groups, namely the amino-tri-acetic acid and the citric acid anions. The additional roles of the nitrogen atom for the first one and of the hydroxy function for the second one are discussed. Accordingly, five new complexes with either americium or lanthanides elements are described: [Co(NH3)6][M(NTA)2(H2O)].8H2O with M Nd, Yb and Am, and [Co(NH3)6]2K[M3(Cit)4(H2O)3].18H2O with Nd and Am cations. In all cases the americium complexes are isostructural with their lanthanide equivalents. (authors)

  11. MARIOS: Irradiation of UO{sub 2} containing 15% americium at well defined temperature

    Energy Technology Data Exchange (ETDEWEB)

    D' Agata, E., E-mail: elio.dagata@ec.europa.eu [European Commission, Joint Research Centre, Institute for Energy - P.O. Box 2, 1755 ZG Petten (Netherlands); Hania, P.R. [Nuclear Research and Consultancy Group, P.O. Box 25, 1755 ZG Petten (Netherlands); Bejaoui, S. [Commissariat a l' Energie Atomique, DEC CEA-Cadarache, 13108 St. Paul lez Durance Cedex (France); Sciolla, C.; Wyatt, T.; Hannink, M.H.C. [Nuclear Research and Consultancy Group, P.O. Box 25, 1755 ZG Petten (Netherlands); Herlet, N.; Jankowiak, A. [Commissariat a l' Energie Atomique DTEC CEA Marcoule, 30207 Bagnols sur Ceze Cedex (France); Klaassen, F.C. [Nuclear Research and Consultancy Group, P.O. Box 25, 1755 ZG Petten (Netherlands); Bonnerot, J.-M. [Commissariat a l' Energie Atomique, DEC CEA-Cadarache, 13108 St. Paul lez Durance Cedex (France)

    2012-01-15

    Highlights: Black-Right-Pointing-Pointer MARIOS is designed to check the behaviour of Minor Actinide Blanket Module concept. Black-Right-Pointing-Pointer Main requirement of the experiment is an accurate control of the temperature. Black-Right-Pointing-Pointer The swelling and the helium release will be the main output of the experiment. Black-Right-Pointing-Pointer A complementary experiment (DIAMINO), will be performed in the next future. - Abstract: Americium is a strong contributor to the long term radiotoxicity of high activity nuclear waste. Transmutation by irradiation in nuclear reactors of long-lived nuclides like {sup 241}Am is, therefore, an option for the reduction of radiotoxicity and residual power packages as well as the repository area. The MARIOS irradiation experiment is the latest of a series of experiments on americium transmutation (e.g. EFTTRA-T4, EFTTRA-T4bis, HELIOS). MARIOS experiment is carried out in the framework of the 4-year project FAIRFUELS of the EURATOM 7th Framework Programme (FP7). During the past years of experimental work in the field of transmutation and tests of innovative nuclear fuel containing americium, the release or trapping of helium as well as swelling has shown to be the key issue for the design of such kinds of target. Therefore, the main objective of the MARIOS experiment is to study the in-pile behaviour of UO{sub 2} containing minor actinides (MAs) in order to gain knowledge on the role of the microstructure and of the temperature on the gas release and on fuel swelling. The MARIOS experiment will be conducted in the HFR (high flux reactor) in Petten (The Netherlands) and will start in the beginning of 2011. It has been planned that the experiment will last 11 cycles, corresponding to 11 months. This paper covers the description of the objective of the experiment, as well as a general description of the design of the experiment.

  12. Speciation of americium in seawater and accumulation in the marine sponge Aplysina cavernicola.

    Science.gov (United States)

    Maloubier, Melody; Michel, Hervé; Solari, Pier Lorenzo; Moisy, Philippe; Tribalat, Marie-Aude; Oberhaensli, François R; Dechraoui Bottein, Marie Yasmine; Thomas, Olivier P; Monfort, Marguerite; Moulin, Christophe; Den Auwer, Christophe

    2015-12-21

    The fate of radionuclides in the environment is a cause of great concern for modern society, seen especially in 2011 after the Fukushima accident. Among the environmental compartments, seawater covers most of the earth's surface and may be directly or indirectly impacted. The interaction between radionuclides and the marine compartment is therefore essential for better understanding the transfer mechanisms from the hydrosphere to the biosphere. This information allows for the evaluation of the impact on humans via our interaction with the biotope that has been largely undocumented up to now. In this report, we attempt to make a link between the speciation of heavy elements in natural seawater and their uptake by a model marine organism. More specifically, because the interaction of actinides with marine invertebrates has been poorly studied, the accumulation in a representative member of the Mediterranean coralligenous habitat, the sponge Aplysina cavernicola, was investigated and its uptake curve exposed to a radiotracer (241)Am was estimated using a high-purity Ge gamma spectrometer. But in order to go beyond the phenomenological accumulation rate, the speciation of americium(III) in seawater must be assessed. The speciation of (241)Am (and natural europium as its chemically stable surrogate) in seawater was determined using a combination of different techniques: Time-Resolved Laser-Induced Fluorescence (TRLIF), Extended X-ray Absorption Fine Structure (EXAFS) at the LIII edge, Attenuated Total Reflectance Fourier Transform Infrared (ATR-FTIR) spectroscopy and Scanning Electron Microscopy (SEM) and the resulting data were compared with the speciation modeling. In seawater, the americium(III) complex (as well as the corresponding europium complex, although with conformational differences) was identified as a ternary sodium biscarbonato complex, whose formula can be tentatively written as NaAm(CO3)2·nH2O. It is therefore this chemical form of americium that is

  13. Speciation of americium in seawater and accumulation in the marine sponge Aplysina cavernicola.

    Science.gov (United States)

    Maloubier, Melody; Michel, Hervé; Solari, Pier Lorenzo; Moisy, Philippe; Tribalat, Marie-Aude; Oberhaensli, François R; Dechraoui Bottein, Marie Yasmine; Thomas, Olivier P; Monfort, Marguerite; Moulin, Christophe; Den Auwer, Christophe

    2015-12-21

    The fate of radionuclides in the environment is a cause of great concern for modern society, seen especially in 2011 after the Fukushima accident. Among the environmental compartments, seawater covers most of the earth's surface and may be directly or indirectly impacted. The interaction between radionuclides and the marine compartment is therefore essential for better understanding the transfer mechanisms from the hydrosphere to the biosphere. This information allows for the evaluation of the impact on humans via our interaction with the biotope that has been largely undocumented up to now. In this report, we attempt to make a link between the speciation of heavy elements in natural seawater and their uptake by a model marine organism. More specifically, because the interaction of actinides with marine invertebrates has been poorly studied, the accumulation in a representative member of the Mediterranean coralligenous habitat, the sponge Aplysina cavernicola, was investigated and its uptake curve exposed to a radiotracer (241)Am was estimated using a high-purity Ge gamma spectrometer. But in order to go beyond the phenomenological accumulation rate, the speciation of americium(III) in seawater must be assessed. The speciation of (241)Am (and natural europium as its chemically stable surrogate) in seawater was determined using a combination of different techniques: Time-Resolved Laser-Induced Fluorescence (TRLIF), Extended X-ray Absorption Fine Structure (EXAFS) at the LIII edge, Attenuated Total Reflectance Fourier Transform Infrared (ATR-FTIR) spectroscopy and Scanning Electron Microscopy (SEM) and the resulting data were compared with the speciation modeling. In seawater, the americium(III) complex (as well as the corresponding europium complex, although with conformational differences) was identified as a ternary sodium biscarbonato complex, whose formula can be tentatively written as NaAm(CO3)2·nH2O. It is therefore this chemical form of americium that is

  14. Americium characterization by X-ray fluorescence and absorption spectroscopy in plutonium uranium mixed oxide

    International Nuclear Information System (INIS)

    Plutonium uranium mixed oxide (MOX) fuels are currently used in nuclear reactors. The actinides in these fuels need to be analyzed after irradiation for assessing their behaviour with regard to their environment and the coolant. In this work the study of the atomic structure and next-neighbour environment of Am in the (Pu,U)O2 lattice in an irradiated (60 MW d kg−1) MOX sample was performed employing micro-X-ray fluorescence (µ-XRF) and micro-X-ray absorption fine structure (µ-XAFS) spectroscopy. The chemical bonds, valences and stoichiometry of Am (∼0.66 wt%) are determined from the experimental data gained for the irradiated fuel material examined in its peripheral zone (rim) of the fuel. In the irradiated sample Am builds up as Am3+ species within an [AmO8]13− coordination environment (e.g. >90%) and no (III XAFS spectra recorded for the irradiated MOX sub-sample in the rim zone for a 300 μm×300 μm beam size area investigated over six scans of 4 h. The records remain constant during multi-scan. The analysis of the XAFS signal shows that Am is found as trivalent in the UO2 matrix. This analytical work shall open the door of very challenging analysis (speciation of fission product and actinides) in irradiated nuclear fuels. - Highlights: • Americium was characterized by microX-ray absorption spectroscopy in irradiated MOX fuel. • The americium redox state as determined from XAS data of irradiated fuel material was Am(III). • In the sample, the Am3+ face an AmO813− coordination environment in the (Pu,U)O2 matrix. • The americium dioxide is reduced by the uranium dioxide matrix

  15. Fabrication of uranium–americium mixed oxide pellet from microsphere precursors: Application of CRMP process

    Energy Technology Data Exchange (ETDEWEB)

    Remy, E. [Radiochemistry and Processes Department, CEA, Nuclear Energy Division, F-30207 Bagnols-sur-Cèze (France); Picart, S., E-mail: sebastien.picart@cea.fr [Radiochemistry and Processes Department, CEA, Nuclear Energy Division, F-30207 Bagnols-sur-Cèze (France); Delahaye, T. [Fuel Cycle Technology Department, CEA, Nuclear Energy Division, F-30207 Bagnols-sur-Cèze (France); Jobelin, I. [Radiochemistry and Processes Department, CEA, Nuclear Energy Division, F-30207 Bagnols-sur-Cèze (France); Lebreton, F.; Horlait, D. [Fuel Cycle Technology Department, CEA, Nuclear Energy Division, F-30207 Bagnols-sur-Cèze (France); Bisel, I. [Radiochemistry and Processes Department, CEA, Nuclear Energy Division, F-30207 Bagnols-sur-Cèze (France); Blanchart, P. [Heterogeneous Materials Research Group, Centre Européen de la Céramique, F-87068 Limoges (France); Ayral, A. [Institut Européen des Membranes, CNRS-ENSCM-UM2, CC47, University Montpellier 2, F-34095 Montpellier cedex 5 (France)

    2014-10-15

    Highlights: • Dust free process for (U,Am)O{sub 2} transmutation target fabrication. • Synthesis of U{sub 0.9}Am{sub 0.1}O{sub 2} mixed oxide microspheres from ion exchange resin. • Fabrication of dense U{sub 0.9}Am{sub 0.1}O{sub 2} pellet with 95% TD from mixed oxide microspheres. - Abstract: Mixed uranium–americium oxides are one of the materials envisaged for Americium Bearing Blankets dedicated to transmutation in fast neutron reactors. Recently, several processes have been developed in order to validate fabrication flowchart in terms of material specifications such as density and homogeneity but also to suggest simplifications for lowering industrial costs and hazards linked to dust generation of highly contaminating and irradiating compounds. This study deals with the application of an innovative route using mixed oxide microspheres obtained from metal loaded resin bead calcination, called Calcined Resin Microsphere Pelletization (CRMP). The synthesis of mixed oxide microsphere precursor of U{sub 0.9}Am{sub 0.1}O{sub 2±δ} is described as well as its characterisation. The use of this free-flowing precursor allows the pressing and sintering of one pellet of U{sub 0.9}Am{sub 0.1}O{sub 2±δ}. The ceramic obtained was characterised and results showed that its microstructure is dense and homogeneous and its density attains 95% of the theoretical density. This study validates the scientific feasibility of the CRMP process applied to the fabrication of uranium and americium-containing materials.

  16. Influence of biofilms on migration of uranium, americium and europium in the environment

    International Nuclear Information System (INIS)

    The report on the influence of biofilms on migration of uranium, americium and europium in the environment deals with the contamination problems of uranium mines such as SDAG WISMUT in Saxonia and Thuringia. In mine waters microorganisms form a complex microbiological biocoenosis in spite of low pH values and high heavy metal concentrations including high uranium concentrations. The analyses used microbiological methods like confocal laser scanning microscopy and molecular-biological techniques. The interactions of microorganism with fluorescent radioactive heavy metal ions were performed with TRLFS (time resolved laser-induced fluorescence spectroscopy).

  17. Plutonium and americium in arctic waters, the North Sea and Scottish and Irish coastal zones

    DEFF Research Database (Denmark)

    Hallstadius, L.; Aarkrog, Asker; Dahlgaard, Henning;

    1986-01-01

    Plutonium and americium have been measured in surface waters of the Greenland and Barents Seas and in the northern North Sea from 1980 through 1984. Measurements in water and biota, Fucus, Mytilus and Patella, were carried out in North-English and Scottish waters in 1982 and Fucus samples were...... plutonium from the latter to Spitsbergen waters. Fallout plutonium in Arctic waters has a residence time of the order of several years, while for Pu from Sellafield we estimate mean residence times of 11–15 months in Scottish waters and, tentatively, 1·5-3 y during transport from the North Channel (north...

  18. Comparison of acid leachate and fusion methods to determine plutonium and americium in environmental samples

    International Nuclear Information System (INIS)

    The Analytical Chemistry Laboratory at Argonne National Laboratory performs radiochemical analyses for a wide variety of sites within the Department of Energy complex. Since the chemical history of the samples may vary drastically from site to site, the effectiveness of any analytical technique may also vary. This study compares a potassium fluoride-pyrosulfate fusion technique with an acid leachate method. Both normal and high-fired soils and vegetation samples were analyzed for both americium and plutonium. Results show both methods work well, except for plutonium in high-fired soils. Here the fusion method provides higher accuracy

  19. Purification of used scintillation liquids containing the alpha emitters americium and plutonium

    International Nuclear Information System (INIS)

    In Sweden, alpha radioactive waste liquids with an activity over some kBq per waste container cannot be sent for final storage. Therefore, in this work, a method for a purification of alpha active scintillation cocktails was developed. Until today (March, 2013) more than 20 L of scintillation liquids have successfully been purified from americium and plutonium. The products of the process are a solid fraction that can be sent to final storage and a practically non-radioactive liquid fraction that can be sent to municipal incineration. (author)

  20. Study of the extraction and the purification of americium and trivalent actinides contained in effluents with supported liquid membranes

    International Nuclear Information System (INIS)

    The supported liquid membrane technique is studied and developed for americium recovery from uranium or plutonium matrices and decontamination of liquid radioactive wastes. First tests on uranium-nickel solutions with a flat membrane showed the easiness of the operation and the efficiency of the process. Acid-resistant (10 N), interchangeable elements with hollow fibers, are developed and also a computerized automatic device. The different tests on americium solutions demonstrate the feasibility and the reliability of the system. Influence of various parameters on transfer kinetics is investigated

  1. Contribution to the prediction of americium, plutonium and neptunium behaviour in the geosphere: chemical data

    International Nuclear Information System (INIS)

    An exhaustive bibliographic review on hydrolysis of americium gives the stability constants, at zero ionic strength. No evidence of Am(OH)4- formation was found by solubility studies up to pH 2 (CO3)3 characterised by its X-ray diffraction pattern is studied at a high ionic strength. All the published results on Am in carbonate media are reinterpreted using these stability constants (Am-OH-CO3 complexes are not needed). No evidence of Am(CO3)45- formation was found by spectrophotometry up to 3M. Literature results are used to determine the formal redox potentials at pH = 9.4 and to calculate the formation constants, at zero ionic strength. The formation of complexes between americium and humic materials (purified fulvic and humic acids) has been studied by a spectrophotometric technique. The results are interpreted by the formation of a 1:1 complexe. Solubility of the solid PuO2(CO3) is measured in bicarbonate media at high ionic strength, to obtain the solubility product and formation constants of the PuO2(CO3)i2-2i complexes

  2. The distribution of plutonium-239 and americium-241 in the Syrian hamster following its intravenous administration as citrate

    International Nuclear Information System (INIS)

    Actinide distribution in various tissues and the skeleton of hamsters by liquid scintillation counting or isotope dilution. For plutonium 57% of activity was concentrated in the skeleton and more than 90% in the liver and skeleton after seven days. For americium the liver retained more than 50% of total activity and 25% was excreted in urine within seven days. (U.K.)

  3. EURADOS intercomparison on measurements and Monte Carlo modelling for the assessment of Americium in a USTUR leg phantom

    International Nuclear Information System (INIS)

    A collaboration of the EURADOS working group on 'Internal Dosimetry' and the United States Transuranium and Uranium Registries (USTUR) has taken place to carry out an intercomparison on measurements and Monte Carlo modelling determining americium deposited in the bone of a USTUR leg phantom. Preliminary results and conclusions of this intercomparison exercise are presented here. (authors)

  4. Anomalous aryl strengthening of americium and europium complexes during extraction by alkylenediphosphine dioxides from perchloric acid media

    International Nuclear Information System (INIS)

    Extraction of americium and europium from perchlorate environments by solutions of three types of methylenediphosphine dioxides, namely (C6H5)P(O)(CH2)sub(n)(O)P(C6H5)2, (C6H5)2P(O)CH2(O)P(C8H17)2 and (C8H17)2P(O)(CH2)sub(n)(O)P(C8H17)2 has been studied (n is 1 or 2 ) The diluents used have been dichlorethane and chloroform. In perchlorate environments the distribuiton coefficients of americium and europium have proved to be by about 3 orders of magnitude higher than in nitric acid environments, i.e. in perchlorate media the complexes are far more stable. Separation coefficients of americium and REE in perchloric acid soutions are much higher than in nitrate environments. The average value of Am/Eu separation coeffecient at 1-5 M acidity was about 6 (with dichlorethane as diluent) or about 7 (with chloroform as diluent). The complexes essentially exist as trisolvated. Americium complexes display anomalous stability increase upon being diluted: by about 2 orders of magnitude with dichlorethane and by up to 3 orders of magnitude with chloroform used as diluent

  5. Investigations of neutron characteristics for salt blanket models; integral fission cross section measurements of neptunium, plutonium, americium and curium isotopes

    International Nuclear Information System (INIS)

    Neutron characteristics of salt blanket micromodels containing eutectic mixtures of sodium, zirconium, and uranium fluorides were measured on FKBN-2M, BIGR and MAKET facilities. The effective fission cross sections of neptunium, plutonium, americium, and curium isotopes were measured on the neutron spectra formed by micromodels. (author)

  6. USB-RS 232转换卡的设计与实现%Design and Realization 0f USB-RS232 Converter Card

    Institute of Scientific and Technical Information of China (English)

    赖彪; 金海鹰; 贾惠芹

    2011-01-01

    与RS 232总线的数据传输速率相比,USB的传输速率高迭480 Mb/s,因此很多计算机的RS 232串行接口都被USB接口所替换,但是很多仪器仪表、控制终端、远程终端等设备的接口还是沿用RS 232.为解决两个接口之间的转换,设计并研制了USB-RS 232接口转换卡.从USB和RS 232通信协议出发,详细介绍USB-RS 232转换卡的设计原理,并以CH341T芯片为例,设计并制作了USB-RS 232转换卡.利用研制的USB-RS 232转换卡连接具有RS 232接口的温湿度传感器,在运行监控程序后,传感器运行稳定,能正确显示温湿度数据,且表明该转换卡可成功地实现RS 232接口与USB接口的转换.%Compared with RS232 bus.USB (universal serial bus) transfer rate can arrive at 480 Mbps.Therefore, many RS232 serial interface has been replaced by USB interface recently, but the RS232 serial interface is still reserved in some equipments, such as instruments, controllers and remote ternunals.A USB-RS232 converter card is designed and realized with CH341T chip to solve this conversion problem between USB and RS-232 bus.The principle of USB-RS232 converter card is discussed in this paper through studying the USB and RS232 protocol.USB-RS232 converter card can be connected with a temperature-humidity sensor through a RS232 interface.The testing result shows that USB-RS232 converter card runs normally, can display the temperature and humidity data correctly, and the design principle of USB-RS232 converter card is correct.

  7. Purification of scintillation cocktails containing the alpha emitters americium and plutonium

    International Nuclear Information System (INIS)

    One efficient way of measuring alpha emitters is by the usage of liquid scintillation counting (LSC). A liquid sample is placed in a vial containing a scintillation cocktail. The alpha particles excite electrons in the surrounding liquid, and when they are de-excited photons are emitted. The photons are detected and the activity can be quantified. LSC has a high efficiency for alpha radiation and is therefore a fast and easy way for measuring alpha emitting samples. One drawback is that it does not differentiate very well between alpha energies; measurements of for example curium and plutonium simultaneously are impossible and demand other techniques. Another drawback is the production of a liquid alpha active waste. In Sweden alpha radioactive waste liquids with an activity over some kBq per waste container cannot be sent for final storage. If, however, the activity of the liquids could be reduced by precipitation of the actinides, it would be possible to send away the liquid samples to municipal incineration. In this work a method for a purification of alpha active scintillation cocktails was developed. The method was first tried on a lab scale, and then scaled up. Until today (March, 2013) more than 20 liters of scintillation liquids have successfully been purified from americium and plutonium at Chalmers University of Technology in Sweden. The four scintillation cocktails used were Emulsifier Safe®, Hionic-Fluor®, Ultima Gold AB® and Ultima Gold XR®. The scintillation cocktails could all be purified from americium with higher yield than 95%. The yield was kept when the liquids were mixed. Also plutonium could be precipitated with a yield over 95% in all cocktails except in Hionic-Fluor® (>55%). However, that liquid in particular could be purified (>95%) by mixing it with the three other cocktails. Up-scaling was performed to a batch size of 6-8 L of scintillation cocktail. In neither the americium nor the plutonium system, adverse effects of increasing the

  8. A thermodynamic study of actinide oxide targets/fuels for americium transmutation

    International Nuclear Information System (INIS)

    A thermodynamic study was performed on the systems Am-O, AmOx-MgO, AmOx-MgAl2O4, Pu-Mg-O and U-Mg-O. Both experimental work (X-ray analyses, oxygen potential measurements etc.) and calculations on the phase diagrams involved were made. The reaction between americium oxide and spinel is expected to form the compound AmAlO3. Isothermal sections have been calculated for AmOx-(MgO, Al2O3), Pu-Mg-O and U-Mg-O at 2000 K using the software package ''Thermo-Calc''. Thermodynamic equilibrium data were used to predict the behaviour of actinide oxides in a reactor. The implication of the results for the technological application is discussed, with emphasis on the effects of the high oxygen potential of AmO2 as compared to the conventional fuel, i.e. UO2. (author)

  9. The uptake of plutonium-239, 240, americium-241, strontium-90 into plants

    International Nuclear Information System (INIS)

    This report describes the results of measurements on the uptake of plutonium, americium, strontium-90 and caesium-137 into peas, beet, oats, sweet corn, tomatoes and vegetable marrow grown in tubs containing radioactively-contaminated silts. The silts had been taken from an area of West Cumbria commonly referred to as the Ravenglass estuary. The experiments are categorised as being carried out under non-standard conditions because of the manner in which the radioactivity came to be incorporated into the growth medium. The growth medium was representative of conditions which could arise when the estuarine silt moves inland under the influence of wind and tide and mixes with the adjacent farm land. The silt had been contaminated by radioactive effluents from the nuclear fuels reprocessing plant at Sellafield and this contamination had been brought about by natural means. (Auth.)

  10. Complex formation of trivalent americium with salicylic acid at very low concentrations

    International Nuclear Information System (INIS)

    For the first time, the complexation of americium(III) with salicylic acid was studied at trace metal concentrations using a 2.0 m Long Path Flow Cell for UV-vis spectroscopy. The detection limit of Am(III) in aqueous solution at pH 3.0 was found to be 5 x 10-9 M. Two Am(III)-salicylate complexes were formed at pH 5.0 in 0.1 M NaClO4, indicated by a clear red shift of the absorption maximum. The absorption spectra obtained from spectrophotometric titration were analyzed by means of factor analysis and complex stabilities were calculated to be log β110 = 2.56 ± 0.08 and log β120 = 3.93 ± 0.19. (author)

  11. Standard practice for The separation of americium from plutonium by ion exchange

    CERN Document Server

    American Society for Testing and Materials. Philadelphia

    2001-01-01

    1.1 This practice describes the use of an ion exchange technique to separate plutonium from solutions containing low concentrations of americium prior to measurement of the 241Am by gamma counting. 1.2 This practice covers the removal of plutonium, but not all the other radioactive isotopes that may interfere in the determination of 241Am. 1.3 This practice can be used when 241Am is to be determined in samples in which the plutonium is in the form of metal, oxide, or other solid provided that the solid is appropriately sampled and dissolved (See Test Methods C758, C759, and C1168). 1.4 This standard does not purport to address all of the safety concerns, if any, associated with its use. It is the responsibility of the user of this standard to establish appropriate safety and health practices and determine the applicability of regulatory limitations prior to use.

  12. Transportability Class of Americium in K Basin Sludge under Ambient and Hydrothermal Processing Conditions

    Energy Technology Data Exchange (ETDEWEB)

    Delegard, Calvin H.; Schmitt, Bruce E.; Schmidt, Andrew J.

    2006-08-01

    This report establishes the technical bases for using a ''slow uptake'' instead of a ''moderate uptake'' transportability class for americium-241 (241Am) for the K Basin Sludge Treatment Project (STP) dose consequence analysis. Slow uptake classes are used for most uranium and plutonium oxides. A moderate uptake class has been used in prior STP analyses for 241Am based on the properties of separated 241Am and its associated oxide. However, when 241Am exists as an ingrown progeny (and as a small mass fraction) within plutonium mixtures, it is appropriate to assign transportability factors of the predominant plutonium mixtures (typically slow) to the Am241. It is argued that the transportability factor for 241Am in sludge likewise should be slow because it exists as a small mass fraction as the ingrown progeny within the uranium oxide in sludge. In this report, the transportability class assignment for 241Am is underpinned with radiochemical characterization data on K Basin sludge and with studies conducted with other irradiated fuel exposed to elevated temperatures and conditions similar to the STP. Key findings and conclusions from evaluation of the characterization data and published literature are summarized here. Plutonium and 241Am make up very small fractions of the uranium within the K Basin sludge matrix. Plutonium is present at about 1 atom per 500 atoms of uranium and 241Am at about 1 atom per 19000 of uranium. Plutonium and americium are found to remain with uranium in the solid phase in all of the {approx}60 samples taken and analyzed from various sources of K Basin sludge. The uranium-specific concentrations of plutonium and americium also remain approximately constant over a uranium concentration range (in the dry sludge solids) from 0.2 to 94 wt%, a factor of {approx}460. This invariability demonstrates that 241Am does not partition from the uranium or plutonium fraction for any characterized sludge matrix. Most

  13. 48 CFR 3452.232-71 - Incremental funding.

    Science.gov (United States)

    2010-10-01

    ... 48 Federal Acquisition Regulations System 7 2010-10-01 2010-10-01 false Incremental funding. 3452... 3452.232-71 Incremental funding. As prescribed in 3452.771, insert the following provision in solicitations: Incremental Funding (AUG 1987) (a) Sufficient funds are not presently available to cover...

  14. 48 CFR 53.232 - Contract financing (SF 1443).

    Science.gov (United States)

    2010-10-01

    ... 48 Federal Acquisition Regulations System 2 2010-10-01 2010-10-01 false Contract financing (SF... (CONTINUED) CLAUSES AND FORMS FORMS Prescription of Forms 53.232 Contract financing (SF 1443). SF 1443 (JUL 2009), Contractor's Request for Progress Payment. SF 1443 is prescribed for use in...

  15. 46 CFR 232.6 - Financial report filing requirement.

    Science.gov (United States)

    2010-10-01

    ... RELATED ACTIVITIES UNIFORM FINANCIAL REPORTING REQUIREMENTS Income Statement § 232.6 Financial report filing requirement. (a) Reporting Frequency and Due Dates. The contractor shall file a semiannual... generally accepted accounting principles and modified to the extent necessary to comply with this...

  16. 48 CFR 232.606 - Debt determination and collection.

    Science.gov (United States)

    2010-10-01

    ... SYSTEM, DEPARTMENT OF DEFENSE GENERAL CONTRACTING REQUIREMENTS CONTRACT FINANCING Contract Debts 232.606 Debt determination and collection. When transferring a case to the contract financing office, follow... 48 Federal Acquisition Regulations System 3 2010-10-01 2010-10-01 false Debt determination...

  17. Estimated Release of Tritium from 232-F Concrete Rubble

    International Nuclear Information System (INIS)

    This report describes an estimate of the release of tritium from contaminated concrete from the demolition of the old 232-F Tritium Facility at the Savannah River Site. The estimate uses data from the scientific literature and information about tritium migration in concrete developed during studies of tritium in concrete at SRS

  18. 17 CFR 232.301 - EDGAR Filer Manual.

    Science.gov (United States)

    2010-04-01

    ... the Federal Register in accordance with 5 U.S.C. 552(a) and 1 CFR part 51. You must comply with these... 17 Commodity and Securities Exchanges 2 2010-04-01 2010-04-01 false EDGAR Filer Manual. 232.301... Filer Manual. Filers must prepare electronic filings in the manner prescribed by the EDGAR Filer...

  19. 24 CFR 232.570 - Endorsement of credit instrument.

    Science.gov (United States)

    2010-04-01

    ... 24 Housing and Urban Development 2 2010-04-01 2010-04-01 false Endorsement of credit instrument... of Fire Safety Equipment Eligible Security Instruments § 232.570 Endorsement of credit instrument. The Commissioner shall indicate his insurance of the loan by endorsing the credit instrument...

  20. Preparation of 232Th Target by Molecule Plating

    Institute of Scientific and Technical Information of China (English)

    2008-01-01

    <正>For the cross section measurement of the 232Th(α, 2n)234U reaction, thorium targets plated on the aluminium foil with 2 and 8 μm thickness are required. It was demanded that the mass thickness of the

  1. 17 CFR 232.12 - Business hours of the Commission.

    Science.gov (United States)

    2010-04-01

    ... REGULATION S-T-GENERAL RULES AND REGULATIONS FOR ELECTRONIC FILINGS General § 232.12 Business hours of the... 17 Commodity and Securities Exchanges 2 2010-04-01 2010-04-01 false Business hours of the..., whichever is currently in effect. (c) Submissions by direct transmission. Electronic filings and...

  2. 17 CFR 232.201 - Temporary hardship exemption.

    Science.gov (United States)

    2010-04-01

    ... no later than one business day after the date on which the filing was to be made. (1) An electronic... submitted to the Commission within six business days of filing the paper format document. The electronic... REGULATION S-T-GENERAL RULES AND REGULATIONS FOR ELECTRONIC FILINGS Hardship Exemptions § 232.201...

  3. 24 CFR 232.903 - Maximum mortgage limitations.

    Science.gov (United States)

    2010-04-01

    ... to be refinanced by the insured mortgage (i.e., without a change of ownership or with the Project sold to a purchaser who has an identity of interest as defined by the Commissioner with the seller with..., organizational, title, and recording expenses, including mortgagee fees under § 232.15; (4) The estimated...

  4. 48 CFR 3452.232-72 - Method of payment.

    Science.gov (United States)

    2010-10-01

    ... 48 Federal Acquisition Regulations System 7 2010-10-01 2010-10-01 false Method of payment. 3452... 3452.232-72 Method of payment. As prescribed in 3432.170, insert the following clause in all solicitations and contracts: Method of Payment (AUG 1987) (a) Payments under this contract will be made...

  5. Benchmarking ~(232)Th Evaluations With KBR and Thor Experiments

    Institute of Scientific and Technical Information of China (English)

    2011-01-01

    The n+232Th evaluations from CENDL-3.1, ENDF/B-Ⅶ.0, JENDL-3.3 and JENDL-4.0 were tested with KBR series and THOR benchmark from ICSBEP Handbook. THOR is Plutonium-Metal-Fast (PMF) criticality benchmark reflected with metal thorium.

  6. Determination of uranium isotopes in urine samples from radiation workers using 232U tracer, anion-exchange resin and alpha-spectrometry

    International Nuclear Information System (INIS)

    Bioassay technique is used for the estimation of actinides present in the body based on the excretion rate of body fluids. For occupational radiation workers urine assay is the preferred method for monitoring of chronic internal exposure. Determination of low concentrations of actinides such as plutonium, americium and uranium at low level of mBq in urine by alpha-spectrometry requires pre-concentration of large volumes of urine. This paper deals with standardization of analytical method for the determination of U-isotopes in urine samples using anion-exchange resin and 232U tracer for radiochemical recovery. The method involves oxidation of urine followed by co-precipitation of uranium along with calcium phosphate. Separation of U was carried out by Amberlite, IRA-400, anion-exchange resin. U-fraction was electrodeposited and activity estimated using tracer recovery by alpha-spectrometer. Eight routine urine samples of radiation workers were analyzed and consistent radiochemical tracer recovery was obtained in the range of 51% to 67% with a mean and standard deviation of 60% and 5.4%, respectively. (author)

  7. Simulation calculation of 232U productions in thorium-uranium transform process based on thermal reactor

    International Nuclear Information System (INIS)

    The decay products of 232U produced in the thorium-uranium fuel cycle emit high energy γ-rays. This affects the fuel cycle greatly. In this paper, the 232U productions in thermal reactor using thorium fuel are analyzed by ORIGEN2, SCALE5 and the code based on the Bateman method. Under normal situation, 232U is mainly produced by 232Th (n, 2n) reaction chain, and more quantity of 230Th can be transformed into 232U while the neutron spectrum is softer. The burnup calculation of CANDU reactor and PWR assembly indicates that the 232U in uranium increase with the burnup, and 230Th in fresh thorium has linear correlation with 232U/Utotal or 232U/233U at discharge burnup. (authors)

  8. 49 CFR 232.207 - Class IA brake tests-1,000-mile inspection.

    Science.gov (United States)

    2010-10-01

    ... 49 Transportation 4 2010-10-01 2010-10-01 false Class IA brake tests-1,000-mile inspection. 232... Class IA brake tests—1,000-mile inspection. (a) Except as provided in § 232.213, each train shall receive a Class IA brake test performed by a qualified person, as defined in § 232.5, at a location...

  9. 48 CFR 552.232-77 - Payment By Government Charge Card.

    Science.gov (United States)

    2010-10-01

    ... 48 Federal Acquisition Regulations System 4 2010-10-01 2010-10-01 false Payment By Government Charge Card. 552.232-77 Section 552.232-77 Federal Acquisition Regulations System GENERAL SERVICES ADMINISTRATION CLAUSES AND FORMS SOLICITATION PROVISIONS AND CONTRACT CLAUSES Text of Provisions and Clauses 552.232-77 Payment By Government Charge...

  10. 36 CFR 223.232 - Disclosure of relation to other bidders.

    Science.gov (United States)

    2010-07-01

    ... 36 Parks, Forests, and Public Property 2 2010-07-01 2010-07-01 false Disclosure of relation to other bidders. 223.232 Section 223.232 Parks, Forests, and Public Property FOREST SERVICE, DEPARTMENT OF... § 223.232 Disclosure of relation to other bidders. The Forest Service may require any prospective...

  11. 25 CFR 1000.232 - When must DOI respond to a request for reconsideration?

    Science.gov (United States)

    2010-04-01

    ... 25 Indians 2 2010-04-01 2010-04-01 false When must DOI respond to a request for reconsideration? 1000.232 Section 1000.232 Indians OFFICE OF THE ASSISTANT SECRETARY, INDIAN AFFAIRS, DEPARTMENT OF THE...-DETERMINATION AND EDUCATION ACT Waiver of Regulations § 1000.232 When must DOI respond to a request...

  12. 43 CFR 2.32 - How long does DOI have to respond to my appeal?

    Science.gov (United States)

    2010-10-01

    ... 43 Public Lands: Interior 1 2010-10-01 2010-10-01 false How long does DOI have to respond to my appeal? 2.32 Section 2.32 Public Lands: Interior Office of the Secretary of the Interior RECORDS AND TESTIMONY; FREEDOM OF INFORMATION ACT FOIA Appeals § 2.32 How long does DOI have to respond to my appeal?...

  13. 48 CFR 232.670 - Transfer of responsibility for debt collection.

    Science.gov (United States)

    2010-10-01

    ... for debt collection. 232.670 Section 232.670 Federal Acquisition Regulations System DEFENSE ACQUISITION REGULATIONS SYSTEM, DEPARTMENT OF DEFENSE GENERAL CONTRACTING REQUIREMENTS CONTRACT FINANCING Contract Debts 232.670 Transfer of responsibility for debt collection. Follow the procedures at PGI...

  14. 48 CFR 232.610 - Demand for payment of contract debt.

    Science.gov (United States)

    2010-10-01

    ... contract debt. 232.610 Section 232.610 Federal Acquisition Regulations System DEFENSE ACQUISITION REGULATIONS SYSTEM, DEPARTMENT OF DEFENSE GENERAL CONTRACTING REQUIREMENTS CONTRACT FINANCING Contract Debts 232.610 Demand for payment of contract debt. When issuing a demand for payment of a contract...

  15. 48 CFR 232.006 - Reduction or suspension of contract payments upon finding of fraud.

    Science.gov (United States)

    2010-10-01

    ... 48 Federal Acquisition Regulations System 3 2010-10-01 2010-10-01 false Reduction or suspension of contract payments upon finding of fraud. 232.006 Section 232.006 Federal Acquisition Regulations System... FINANCING 232.006 Reduction or suspension of contract payments upon finding of fraud....

  16. 22 CFR 23.2 - Endorsing remittances for deposit in the Treasury.

    Science.gov (United States)

    2010-04-01

    ... 22 Foreign Relations 1 2010-04-01 2010-04-01 false Endorsing remittances for deposit in the Treasury. 23.2 Section 23.2 Foreign Relations DEPARTMENT OF STATE FEES AND FUNDS FINANCE AND ACCOUNTING § 23.2 Endorsing remittances for deposit in the Treasury. The Office of Finance—Cashier Unit,...

  17. 49 CFR 232.603 - Design, interoperability, and configuration management requirements.

    Science.gov (United States)

    2010-10-01

    ... management requirements. 232.603 Section 232.603 Transportation Other Regulations Relating to Transportation... Pneumatic (ECP) Braking Systems § 232.603 Design, interoperability, and configuration management requirements. (a) General. A freight car or freight train equipped with an ECP brake system shall, at a...

  18. The behaviour under irradiation of molybdenum matrix for inert matrix fuel containing americium oxide (CerMet concept)

    Science.gov (United States)

    D'Agata, E.; Knol, S.; Fedorov, A. V.; Fernandez, A.; Somers, J.; Klaassen, F.

    2015-10-01

    Americium is a strong contributor to the long term radiotoxicity of high activity nuclear waste. Transmutation by irradiation in nuclear reactors or Accelerator Driven System (ADS, subcritical reactors dedicated to transmutation) of long-lived nuclides like 241Am is therefore an option for the reduction of radiotoxicity of waste packages to be stored in a repository. In order to safely burn americium in a fast reactor or ADS, it must be incorporated in a matrix that could be metallic (CerMet target) or ceramic (CerCer target). One of the most promising matrix to incorporate Am is molybdenum. In order to address the issues (swelling, stability under irradiation, gas retention and release) of using Mo as matrix to transmute Am, two irradiation experiments have been conducted recently at the High Flux Reactor (HFR) in Petten (The Netherland) namely HELIOS and BODEX. The BODEX experiment is a separate effect test, where the molybdenum behaviour is studied without the presence of fission products using 10B to "produce" helium, the HELIOS experiment included a more representative fuel target with the presence of Am and fission product. This paper covers the results of Post Irradiation Examination (PIE) of the two irradiation experiments mentioned above where molybdenum behaviour has been deeply investigated as possible matrix to transmute americium (CerMet fuel target). The behaviour of molybdenum looks satisfying at operating temperature but at high temperature (above 1000 °C) more investigation should be performed.

  19. Consideration of the effect of lymph-node deposition upon the measurement of plutonium and americium in the lungs

    International Nuclear Information System (INIS)

    Measurement of an inhaled radionuclide by external photon counting includes quantities which may be contained in lymph nodes, as well as quantities in the lungs. An overestimate of the lung burden can result, if a portion of the radionuclide were present in the lymph nodes. This problem is analyzed with respect to the measurement of inhaled plutonium containing plutonium-241 and americium-241, when americium-241 has been used as a tracer for the plutonium. Equations are derived which yield the amounts of americium and of plutonium in the lungs and in the lymph nodes as a function of time after exposure and for various translocation and retention parameters. Count histories (count profiles) of actual exposure cases are compared with calculated count profiles in order to gain insight into possible values of the translocation and retention parameters. Comparison is also made with calculated count profiles using values of translocation and retention parameters recommended by the International Commission on Radiological Protection (ICRP) for use with the Task Group Lung Model. The magnitude of the possible overestimate (error factor) was calculated for combinations o

  20. HELIOS: the new design of the irradiation of U-free fuels for americium transmutation

    Energy Technology Data Exchange (ETDEWEB)

    D' Agata, E. [European Commission, Joint Research Centre, Institute for Energy, P.O. Box 2, 1755 ZG Petten (Netherlands); Klaassen, F.; Sciolla, C. [Nuclear Research and Consultancy Group, Dept. Life Cycle and Innovations, P.O. Box 25 1755 ZG Petten (Netherlands); Fernandez-Carretero, A. [European Commission, Joint Research Centre, Institute for Transuranium Elements, P.O. Box 2340, 76125 Karlsruhe (Germany); Bonnerot, J.M. [Commissariat a l' Energie Atomique, DEC/SESC/LC2I CEA-Cadarache, 13108 St. Paul lez Durance Cedex (France)

    2009-06-15

    Americium is one of the radioactive elements that mostly contribute to the radiotoxicity of the nuclear spent fuel. Transmutation of long-lived nuclides like Americium is an option for the reduction of the mass, the radiotoxicity and the decay heat of nuclear waste. The HELIOS irradiation experiment is the last evolution in a series of experiments on americium transmutation. The previous experiments, EFTTRA-T4 and T4bis, have shown that the release or trapping of helium is the key issue for the design of such kind of target. In fact, the production of helium, which is characteristic of {sup 241}Am transmutation, is quite significant. The experiment is carried out in the framework of the 4-year project EUROTRANS of the EURATOM 6. Framework Programme (FP6). Therefore, the main objective of the HELIOS experiment is to study the in-pile behaviour of U-free fuels such as CerCer (Pu, Am, Zr)O{sub 2} and Am{sub 2}Zr{sub 2}O{sub 7}+MgO or CerMet (Pu, Am)O{sub 2}+Mo in order to gain knowledge on the role of the fuel microstructure and of the temperature on the gas release and on the fuel swelling. The experiment was planned to be conducted in the HFR (High Flux Reactor) in Petten (The Netherlands) starting the first quarter of 2007. Because of the innovative aspects of the fuel, the fabrication has had some delays as well as the final safety analyses of the original design showed some unexpected deviation. Besides, the HFR reactor has been unavailable since August 2008. Due to the reasons described above, the experiment has been postponed. HELIOS should start in the first quarter of 2009 and will last 300 full power days. The paper will cover the description of the new design of the irradiation experiment HELIOS. The experiment has been split in two parts (HELIOS1 and HELIOS2) which will be irradiated together. Moreover, due to the high temperature achieved in cladding and to the high amount of helium produced during transmutation the experiment previously designed for a

  1. Anomalous aryl strengthening of complexes at americium and europium extraction with alkylenediphospine dioxide from perchloric media

    International Nuclear Information System (INIS)

    Studied was the extraction of americium(3) and europium(3) from perchlorate solutions(0.001 M) with dioxides of alkylenediphosphines of three types: aryl Ph2P(O)CH2(O)PPh2(briefly 4P), and Ph2P(O)(CH2)2(O)PPh2, mixed Ph2P(O)CH2(O)P(C8H17)2 (or 2Ph2Oct) and alkyl (C8H17)2P(O)CH2(O)P(C8H17)2 (or 4 Oct). Trisolvates of MeS3x(ClO4)3 are predominantly formed but americium disolvates are also present upon dilution with dichloroethane. For 4Ph,2Ph2Oct and 4 Oct the concentration is, respectively, 1015, 2x1014, and 1013; for disolvates by 4 orders of magnitude lower which is, nevertheless, by 2 orders of magnitude higher than for nitric acid solutions. The separation coefficient of β Am/Eu for 4Ph attains 6-8. As in the case of nitrate solutions, an anomalous aryl strengthening of the complexes is observed: an increase in the distribution coefficients and extraction constants in the series of 4 Oct - 2Ph 2 Oct - 4Ph, in spite of the introduction of electronegative aryl substituents into the dioxide molecule, which reduce electron density on oxygen atoms and basicity of dioxides. In contrast to nitric acid solutions, observed is a nonlinear effect of a change in basicity on extraction properties upon dilution with dichloroethane (dioxide of 2Ph2 Oct does not occupy an intermediate position but is close to 4Ph). Upon dilution with chloroform the dependence is linear and anomalous effect rises due to a different nature of interactions of dioxides with chloroform. When the bridge increases up to ethylene, an anomalous strengthening of the complexes disappears. However, the distribution coefficients upon extraction with alkyl dioxide are considerably lower, which can be explained by a stronger extraction of perchloric acid

  2. Collection and evaluation of nuclear data of Th-232

    International Nuclear Information System (INIS)

    Present status of the requirement to and measurement and evaluation of the nuclear data of Th-232 is presented. The accuracy and energy range of the observed data at present are not enough to the demand from reactor engineering. The data of total cross-section are given in the energy range from 1.5 to 15 MeV from the data by Foster and Fasoli. The data by Uttley for the energy less than 1.5 MeV were accepted. Recently, Whalen and Kobayashi presented new data. Optical potential parameters were deduced. Re-normalization of the capture cross-sections of Th-232 was made on the basis of the evaluated values by Matsunobu and by Kanda. The values are a little smaller than the values in ENDF/B-4. Fission cross-sections were given by Henkel up to 9 MeV, and by Rago and Pankratov for the energy range above 9 MeV. Recently, Behrens presented new data for wide energy range. The accuracy of the measured cross-sections of inelastic scattering is not enough for reactor design. The accurate values of the cross-sections of (n, 2n) reaction of Th-232 have been demanded. Resonance parameters have been measured for wide energy range. In the energy range of thermal neutrons, the capture cross-section is about 7.4 barn. The characteristics of velocity dependence of the capture cross-section in this range should be investigated. (Kato, T.)

  3. D ampersand D Characterization of the 232-F Old Tritium Facility at the Savannah River Site

    International Nuclear Information System (INIS)

    The 232-F ''Old Tritium Facility'' operated in the 1950s as the first tritium production facility at the Savannah River Site (SRS). In 1957, the 232-F operation ceased with tritium production turned over to a larger, technologically improved facility at SRS. The 232-F Facility was abandoned in 1958 and the process areas have remained contaminated with radiological, hazardous and mixed constituents. Decontamination and decommissioning (D ampersand D) of the 232-F Facility is scheduled to occur in the years 1995-1996. This paper presents the D ampersand D characterization efforts for the 232-F Facility

  4. Americium-based oxides: Dense pellet fabrication from co-converted oxalates

    Energy Technology Data Exchange (ETDEWEB)

    Horlait, Denis; Lebreton, Florent [CEA, DEN, DTEC/SDTC/LEMA, 30207 Bagnols-sur-Cèze (France); Gauthé, Aurélie [CEA, DEN, DRCP/SERA/LCAR, 30207 Bagnols-sur-Cèze (France); Caisso, Marie [CEA, DEN, DTEC/SDTC/LEMA, 30207 Bagnols-sur-Cèze (France); Arab-Chapelet, Bénédicte; Picart, Sébastien [CEA, DEN, DRCP/SERA/LCAR, 30207 Bagnols-sur-Cèze (France); Delahaye, Thibaud, E-mail: thibaud.delahaye@cea.fr [CEA, DEN, DTEC/SDTC/LEMA, 30207 Bagnols-sur-Cèze (France)

    2014-01-15

    Mixed oxides are used as nuclear fuels and are notably envisaged for future fuel cycles including plutonium and minor actinide recycling. In this context, processes are being developed for the fabrication of uranium–americium mixed-oxide compounds for transmutation. The purpose of these processes is not only the compliance with fuel specifications in terms of density and homogeneity, but also the simplification of the process for its industrialization as well as lowering dust generation. In this paper, the use of a U{sub 0.85}Am{sub 0.15}O{sub 2±δ} powder synthesized by oxalate co-conversion as a precursor for dense fuel fabrications is assessed. This study notably focuses on sintering, which yielded pellets up to 96% of the theoretical density, taking advantage of the high reactivity and homogeneity of the powder. As-obtained pellets were further characterized to be compared to those obtained via processes based on the UMACS (Uranium Minor Actinide Conventional Sintering) process. This comparison highlights several advantages of co-converted powder as a precursor for simplified processes that generate little dust.

  5. Study of biosorbents application on the treatment of radioactive liquid wastes with americium-241

    International Nuclear Information System (INIS)

    The use of nuclear energy for many different purposes has been intensified and highlighted by the benefits that it provides. Medical diagnosis and therapy, agriculture, industry and electricity generation are examples of its application. However, nuclear energy generates radioactive wastes that require suitable treatment ensuring life and environmental safety. Biosorption and bioaccumulation represent an emergent alternative for the treatment of radioactive liquid wastes, providing volume reduction and physical state change. This work aimed to study biosorbents for the treatment of radioactive liquid wastes contaminated with americium-241 in order to reduce the volume and change the physical state from liquid to solid. The biosorbents evaluated were Saccharomyces cerevisiae immobilized in calcium alginate beads, inactivated and free cells of Saccharomyces cerevisiae, calcium alginate beads, Bacillus subtilis, Cupriavidus metallidurans and Ochrobactrum anthropi. The results were quite satisfactory, achieving 100% in some cases. The technique presented in this work may be useful and viable for implementing at the Waste Management Laboratory of IPEN - CNEN/SP in short term, since it is an easy and low cost method. (author)

  6. Mutual separation of americium(III) and europium(III) using glycolamic acid and thioglycolamic acid

    Energy Technology Data Exchange (ETDEWEB)

    Suneesh, A.S.; Venkatesan, K.A.; Syamala, K.V.; Antony, M.P.; Vasudeva Rao, P.R. [Indira Gandhi Centre for Atomic Research, Kalpakkam (India). Fuel Chemistry Div.

    2012-07-01

    The extractants, bis(2-ethylhexyl)diglycolamicacid (HDEHDGA) and bis(2-ethylhexy)thiodiglycolamic acid (HDEHSDGA) were synthesized and characterized by {sup 1}H and {sup 13}C NMR, mass and IR spectroscopy. The extraction behaviour of {sup (152+154})Eu(III) and {sup 241}Am(III) from nitric acid medium by a solution of HDEHDGA (or HDEHSDGA) in n-dodecane (n-DD) was studied for the mutual separation of actinides and lanthanides. The effect of various parameters such as the pH, concentrations of HDEHDGA, HDEHSDGA, sodium nitrate, N,N,N',N'-tetrakis(2-pyridylmethyl)ethylenediamine (TPEN) and diethylenetriaminepentaacetic acid (DTPA) on the separation factor (SF) of americium(III) over europium(III) and vice versa was studied, and the conditions needed for the preferential separation were optimised. The results show that HDEHDGA exhibits higher extraction for {sup (152+154)}Eu(III) and HDEHSDGA shows the superior selectivity for {sup 241}Am(III). (orig.)

  7. Determination of plutonium americium and curium in soil samples by solvent extraction with trioctylphosphine oxide

    International Nuclear Information System (INIS)

    A method of Pu, Am and Cm determination in soil samples, which was developed for analyzing samples from territories subjected to radioactive contamination as a result of the Chernobyl accident is described. After preliminary treatment the samples were leached by solution of 7 mol/l HNO23+0.3 mol/l KBrO3 during heating. Pu was isolated by extraction with 0.05 mol TOPO from 7 mol/l HNO3. 144Ce and partially remaining in water phase isotopes of Zr, U and Th were isolated in an extraction-chromatographic column with TOPO and PbO2. Then Am and Cm were extracted by 0.2 mol/l TOPO from solution 1 mol/l HLact+0.07 mol/l DTPA+1 mol/l Al(NO3)3. Alpha-activity of both extracted products was determined in liquid scintillation counter. Chemical yield of plutonium counted to 85±10%, that of americium and curium -75±10%. 17 refs

  8. Development and Testing of an Americium/Lanthanide Separation Flowsheet Using Sodium Bismuthate

    Energy Technology Data Exchange (ETDEWEB)

    Jack Law; Bruce Mincher; Troy Garn; Mitchell Greenhalgh; Nicholas Schmitt; Veronica Rutledge

    2014-04-01

    The separation of Am from the lanthanides and curium is a key step in proposed advanced fuel cycle scenarios. The partitioning and transmutation of Am is desirable to minimize the long-term heat load of material interred in a future high-level waste repository. A separation process amenable to process scale-up remains elusive. Given only subtle chemistry differences within and between the ions of the trivalent actinide and lanthanide series this separation is challenging ; however, higher oxidation states of americium can be prepared using sodium bismuthate and separated via solvent extraction using diamylamylphosphonate (DAAP) extraction. Among the other trivalent metals only Ce is also oxidized and extracted. Due to the long-term instability of Am(VI) , the loaded organic phase is readily selectively stripped to partition the actinide to a new acidic aqueous phase. Batch extraction distribution ratio measurements were used to design a flowsheet to accomplish this separation. Additionally, crossflow filtration was investigated as a method to filter the bismuthate solids from the feed solution prior to extraction. Results of the filtration studies, flowsheet development work and flowsheet performance testing using a centrifugal contactor are detailed.

  9. Speciation and bioavailability of Americium-241 in the fresh water environment

    International Nuclear Information System (INIS)

    Due to its anthropogenic origin, the transuranic americium 241 confronts physiologists with the intriguing question, which mechanisms are involved in the incorporation or elimination of such artificial elements in biological cycles. The investigations on the speciation and bioavailability of 241Am in the freshwater environment aim to establish a relation between the behavior of 241Am in freshwater ecosystems and its availability for biota. In the limnic environment, most often characterized by a high organic load and a low conductivity, the effect of complexation of 241Am with humic acids and competition with trivalent cations such as A1 and Fe, were proven to be significant on the speciation of 241Am. Based on the registration of the 241Am uptake by a large number of freshwater organisms, the crayfish Astacus leptodactylus Eschscholtz was chosen to study the whole-body uptake of 241Am, its corresponding organ distribution and its retention in the animal. The share of external fixation and ingestion in the global uptake, and the effect of speciation on it, were studied more carefully. Other aspects in this physiological part were: the kinetics of 241Am in the hemolymph and the hepatopancreas, and its subcellular distribution in the digestive gland. Finally, by comparing the physiology of 241Am with some other metals (240Pu, 64Cu, 198Au) with analogous or contradictional properties, we tried to find out whether the behavior of 241Am in organisms can be explained from its chemical characteristics

  10. Solution speciation of plutonium and Americium at an Australian legacy radioactive waste disposal site.

    Science.gov (United States)

    Ikeda-Ohno, Atsushi; Harrison, Jennifer J; Thiruvoth, Sangeeth; Wilsher, Kerry; Wong, Henri K Y; Johansen, Mathew P; Waite, T David; Payne, Timothy E

    2014-09-01

    During the 1960s, radioactive waste containing small amounts of plutonium (Pu) and americium (Am) was disposed in shallow trenches at the Little Forest Burial Ground (LFBG), located near the southern suburbs of Sydney, Australia. Because of periodic saturation and overflowing of the former disposal trenches, Pu and Am have been transferred from the buried wastes into the surrounding surface soils. The presence of readily detected amounts of Pu and Am in the trench waters provides a unique opportunity to study their aqueous speciation under environmentally relevant conditions. This study aims to comprehensively investigate the chemical speciation of Pu and Am in the trench water by combining fluoride coprecipitation, solvent extraction, particle size fractionation, and thermochemical modeling. The predominant oxidation states of dissolved Pu and Am species were found to be Pu(IV) and Am(III), and large proportions of both actinides (Pu, 97.7%; Am, 86.8%) were associated with mobile colloids in the submicron size range. On the basis of this information, possible management options are assessed. PMID:25126837

  11. Solution speciation of plutonium and Americium at an Australian legacy radioactive waste disposal site.

    Science.gov (United States)

    Ikeda-Ohno, Atsushi; Harrison, Jennifer J; Thiruvoth, Sangeeth; Wilsher, Kerry; Wong, Henri K Y; Johansen, Mathew P; Waite, T David; Payne, Timothy E

    2014-09-01

    During the 1960s, radioactive waste containing small amounts of plutonium (Pu) and americium (Am) was disposed in shallow trenches at the Little Forest Burial Ground (LFBG), located near the southern suburbs of Sydney, Australia. Because of periodic saturation and overflowing of the former disposal trenches, Pu and Am have been transferred from the buried wastes into the surrounding surface soils. The presence of readily detected amounts of Pu and Am in the trench waters provides a unique opportunity to study their aqueous speciation under environmentally relevant conditions. This study aims to comprehensively investigate the chemical speciation of Pu and Am in the trench water by combining fluoride coprecipitation, solvent extraction, particle size fractionation, and thermochemical modeling. The predominant oxidation states of dissolved Pu and Am species were found to be Pu(IV) and Am(III), and large proportions of both actinides (Pu, 97.7%; Am, 86.8%) were associated with mobile colloids in the submicron size range. On the basis of this information, possible management options are assessed.

  12. Thorium-232 in human tissues: Metabolic parameters and radiation doses

    International Nuclear Information System (INIS)

    Higher than environmental levels of 232Th have been found in autopsy samples of lungs and other organs from four former employees of a Th refinery. Working periods of the subjects ranged from 3 to 24 years, and times from end of work to death ranged from 6 to 31 years. Concentrations of 232Th in these samples and in tissues from two cases of non-occupational exposure were examined for compatibility with dosimetric models in Publication 30 of the International Commission on Radiological Protection (ICPP 1979a). The concentrations of 232Th in the lungs of the Th workers relative to the concentrations in bone or liver were much higher than calculated from the model for class Y aerosols of Th and the exposure histories of the subjects, and concentrations in the pulmonary lymph nodes were much lower than calculated for three of the Th workers and both non-occupational cases. Least-squares fits to the measured concentrations showed that the biological half-times of Th in liver, spleen, and kidneys are similar to the half-time in bone instead of the factor of 10 less suggested in Publication 30, and the fractions translocated from body fluids were found to be about 0.03, 0.02, and 0.005, respectively, when the fraction to bone was held at the suggested value of 0.7. Fitted values of the respiratory parameters differed significantly between cases and the differences were ascribable to aerosol differences. Average inhalation rates calculated for individual Th workers ranged from 50 to 110 Bq 232Th y-1, and dose equivalents as high as 9.3 Sv to the lungs, 2.0 Sv to bone surfaces, and 1.1 Sv effective dose equivalent were calculated from the inhalation rates and fitted values of the metabolic parameters. The radiation doses were about the same when calculated from parameter values fitted with an assumed translocation fraction of 0.2 from body fluids to bone instead of 0.7

  13. PC interfacing using Centronics, RS232 and game ports

    CERN Document Server

    An, Pei

    1998-01-01

    The main links with your PC and the outside world are the centronic port, used for connecting the printer, the RS232 port, used for the mouse, and the games port for a joystick. This book explores how these input/output (I/O) ports can be put to use through a range of other interfacing applications. This is especially useful for laptop and palmtop PCs which cannot be fitted with internal I/O cards. A novel approach is taken by this book, combining the hardware through which the ports can be explored, and the software programming needed to carry out a range of experiments.Circuits are p

  14. A study of plutonium and americium concentrations in seaspray on the southern Scottish coast

    International Nuclear Information System (INIS)

    Seaspray and seawater have been collected from the southern Scottish coast and, for comparison, Cumbria in northwest England during 1989 and 1991. The occurrence of sea-to-land transfer of the actinides plutonium and americium in seaspray was observed on these coasts using muslin screens (a semi-quantitative technique most efficient for collecting large spray droplets) and high volume conventional air samplers. The actinides and fine particulate in the spray were present in relatively higher concentrations than measured in the adjacent seawater, i.e. the spray was enriched in particulate actinides. The net efficiency of the muslim screens in collecting airborne plutonium isotopes and 241Am generally appeared to be about 20%. A review of earlier published concentrations of 239+240Pu and 241Am measured in aerosol and deposition for over a year several tens of metres inland was carried out. This suggested that airborne activities are up to a factor of 5 times higher in Cumbria than southern Scotland. However, neither the new data collected in 1989 and 1991 nor this older data suggests any enhancement of seaspray actinide enrichment in southern Scotland compared to Cumbria. This finding contrasts with earlier, more limited, comparisons that have been carried out which suggested such a difference. There is clear evidence of considerable localised spatial and temporal variability in aerosol actinide enrichment over the beaches in both areas. Enrichments varies between 20 and 500 relative to the adjacent surf zone waters. However, the average enrichment in spray based on the continuous measurements made further inland is likely to be at the lower end of this range. (author)

  15. Biosorption of Americium-242 by saccharomyces cerevisiae: preliminary evaluation and mechanism

    International Nuclear Information System (INIS)

    As an important radioisotope in nuclear industry and other fields, americium-241 is one of the most serious contamination concerns duo to its high radiation toxicity and long half-life. In this experiment, the biosorption of 241Am from solution by a fungus, Saccharomyces cerevisiae (S. cerevisiae), and the effects of various experimental conditions on the biosorption and the mechanism were explored. The preliminary results showed that S. cerevisiae is a very efficient biosorbent. An average of more than 99% of the total 241Am could be removed by S. cerevisiae of 2.1g/L (dry weight) from 241Am solutions of 2.22MBq/L -555 MBq/L (Co). The adsorption equilibrium was achieved within 1 hour and the optimum pH ranged 1-3. The culture times of more than 16 hours were suitable and the efficient adsorption of 241Am by the S. cerevisiae could be noted. The biosorption of 241Am by the decomposed cell wall, protoplasm or cell membrane of S. cerevisiae was same efficient as by the intact fungus, but the some components of S. cerevisiae, such as protein and acylation group had obvious effect on adsorption. When the concentrations of coexistent Eu3+, Nd3+ were 100 times more than that of 241Am, the adsorption rates would drop to 65%. However, most of the investigated acidic ions have no significant influence on the 241Am adsorption but minute change of pH value, while the saturated EDTA can strong inhibit the biosorption of 241Am.. (authors)

  16. Transport of plutonium, americium, and curium from soils into plants by roots

    International Nuclear Information System (INIS)

    For assessing the dose from radionuclides in agricultural products by ingestion it is necessary to know the soil to plant transfer factors. The literature was entirely investigated, in order to judge the size of the soil to plant transfer factors. In total, 92 publications - from 1948 to 1978 -have been evaluated. As result, transfer factors from 10-9 to 10-3 have been found for Plutonium, and from 10-6 to 1 for Americium. For Curium only few data are available in literature. The considerable variation of the measured transfer factors is based on the dependence of these transfer factors from the ion exchange capacity of soils, from the amount of organic materials, from the pH-value, and from the mode of contamination. There are, in any case, contradictory data, although there has been detected a dependence of the transfer factors from these parameters. Chelating agenst increase the transfer factors to approximately 1300. As well, fertilizers have an influence on the size of the transfer factors - however, the relationships have been scarcely investigated. The distribution of actinides within the individual parts of plants has been investigated. The highest concentrations are in the roots; in the plant parts above ground the concentration of actinides decreases considerably. The most inferior transfer factors were measured for the respective seed or fruits. The soil to plant transfer factors of actinides are more dependend on the age of the plants within one growing period. At the beginning of the period, the transfer factor is considerably higher than at the end of this period. With respect to plants with a growing period of several years, correlations are unknown. (orig.)

  17. The treatment of liquid radioactive waste containing Americium by using a cation exchange method

    International Nuclear Information System (INIS)

    A research in the treatment of a liquid radioactive waste containing americium has been done. The liquid radioactive waste used in this research was standard solution of U dan Ce with the initial activity of 100 ppm. The experimental investigation is aimed at a study of the effects of the waste pH, the column dimension of IR-120 cation exchanger which is expressed as L/D, the flow rate of a liquid waste and the influence of thiocyanate as a complex agent against the efficiency of a decontamination for uranium and cerium element. The experiment was done by passing downward the feed of uranium and cerium solution into an IR-120 type of cation exchanger with the L/D of 11.37. From the experimental parameters done in this research where the influence of waste pH was varied from 3 - 8, the geometric column (L/D) 11.37, the liquid flow rate was from 2.5 - 10 ml/m and the thiocyanate concentration was between 100 ppm-500 ppm can be concluded that the optimum operational condition for the ion exchange achieved were the waste pH for uranium = 4 and the waste pH for cerium = 6, the flow rate = 2.5 ml/men. From the given maximum value of DF for uranium = 24 (DE = 95.83%) and of DF for cerium = 40 (DE = 97.5%), it can also be concluded that this investigation is to be continued in order that the greater value of DF/DE can be achieved

  18. Use of radioisotopes in the study of tetracycline analytical application. Extraction of compounds formed between tetracycline and neptunium and americium elements

    International Nuclear Information System (INIS)

    The behavior of tetracycline as complexing agent, in solvent extraction studies of neptunium and americium, using benzyl alcohol as the organic phase, is presented. By using radioactive tracers of 239Np and 241Am the extraction percent of these elements were determined as a function of pH in the absence and in the presence of several masking agents. The influence of shaking time and the use of different types of supporting eletrolytes upon the extraction behavior was also studied. The extraction curves obtained using EDTA as masking agent show that tetracycline can be used for neptunium and americium separation. In this condition neptunium is extracted into the organic phase and americium remains in the aqueous phase. (Author)

  19. Effect of a long-term release of plutonium and americium into an estuarine and coastal sea ecosystem

    International Nuclear Information System (INIS)

    This paper discusses the general problem of speciation of plutonium and americium in aquatic ecosystems and the implications relative to their fate in those systems. The following conclusions were reached: several oxidation states of plutonium coexist in the natural environment; the effect of environmental changes such as pH and Esub(h) values and complexes are probably the cause of these various oxidation states; a clearer definition of the 'concentration factor' should be given in view of the important role the sediments play in supplying plutonium for transfer through the food web. (author)

  20. EFFECT OF COMPOSITION OF SELECTED GROUNDWATERS FROM THE BASIN AND RANGE PROVINCE ON PLUTONIUM, NEPTUNIUM, AND AMERICIUM SPECIATION.

    Science.gov (United States)

    Rees, Terry F.; Cleveland, Jess M.; Nash, Kenneth L.

    1984-01-01

    The speciation of plutonium, neptunium, and americium was determined in groundwaters from four sources in the Basin and Range Province: the lower carbonate aquifer, Nevada Test Site (NTS) (Crystal Pool); alluvial fill, Frenchman Flat, NTS (well 5C); Hualapai Valley, Arizona (Red Lake south well); and Tularosa Basin, New Mexico (Rentfrow well). The results were interpreted to indicate that plutonium and, to a lesser extent, neptunium are least soluble in reducing groundwaters containing a large concentration of sulfate ion and a small concentration of strongly complexing anions. The results further emphasize the desirability of including studies such as this among the other site-selection criteria for nuclear waste repositories.

  1. Microstructure and elemental distribution of americium-containing MOX fuel under the short-term irradiation tests

    International Nuclear Information System (INIS)

    In order to investigate the effect of americium addition to MOX fuels on the irradiation behavior, the 'Am-1' program is being conducted in JAEA. The Am-1 program consists of two short-term irradiation tests of 10-minute and 24-hour irradiations and a steady-state irradiation test. The short-term irradiation tests were successfully completed and the post irradiation examinations (PIEs) are in progress. The PIEs for Am-containing MOX fuels focused on the microstructural evolution and redistribution behavior of Am at the initial stage of irradiation and the results to date are reported. (author)

  2. Development of a methodology for the determination of americium and thorium by ICP-AES and their inter-element effect

    International Nuclear Information System (INIS)

    Due to the scarcity of good quality uranium resources, the growth of nuclear technology in India is dependent on the utilization of the vast thorium resources. Therefore, Advance Heavy Water Reactor is going to acquire significant role in the scenario of Indian nuclear technology, where (Th, Pu)O2 will be utilized as fuel in the outermost ring of the reactor core. This will lead to a complex matrix containing thorium as well as americium, which is formed due to β-decay of plutonium. The amount of americium is dependent on the burn up and the storage time of the Pu based fuels. In the present case, attempt was made to develop a method for the determination of americium as well as thorium by ICP-AES. Two emission lines of americium were identified and calibration curves were established for determination of americium. Though the detection limit of 283.236 nm line (5 ng mL-1) of americium was found to be better than that of 408.930 nm (11 ng mL-1), the former line is significantly interfered by large amount of thorium. Three analytical lines (i.e. 283.242, 283.730 and 401.913 nm) of thorium were identified and calibration curves were established along with their detection limits. It was observed that 283.242 and 401.913 nm line are having similar detection limits (18 and 13 ng mL-1, respectively) which are better than that of 283.730 nm (60 ng mL-1). This can be attributed to the high background of 283.273 nm channel of thorium. The spectral interference study revealed that even small amount of americium has significant contribution on 283.242 nm channel of thorium while the other two channels remain practically unaffected. Considering both these facts, spectral interference and analytical performance (detection limits and sensitivity), it was concluded that 401.913 nm line is the best analytical line out of the three lines for determination of thorium in presence of americium. (author)

  3. Combined procedure using radiochemical separation of plutonium, americium and uranium radionuclides for alpha-spectrometry

    International Nuclear Information System (INIS)

    Radiochemical separation of Pu, Am and U was tested from synthetic solutions and evaporator concentrate samples from nuclear power plants for isolation of each of them for alpha-spectrometry analysis. The separation was performed by anion-exchange chromatography, extraction chromatography, using TRU resin, and precipitation techniques. The aim of the study was to develop a sensitive analytical procedure for the sequential determination of 242Pu, 238Pu, 239+240Pu, 241Am and 235,238U in radioactive wastes. 238Pu, 242Pu, 243Am and 232U were used as tracers. The measurements of α emitting radionuclides were performed by semiconductor detector that is used especially when spectrometric information is needed. For synthetic solutions the chemical recovery was based on associated iron concentration and was about 93%. (author)

  4. Effect of radiolysis on leachability of plutonium and americium from 76-101 glass. [Glass containing 2 mole % plutonium

    Energy Technology Data Exchange (ETDEWEB)

    Nash, K.L.; Fried, S.; Friedman, A.M.; Susak, N.; Rickert, P.; Sullivan, J.C.; Karim, D.P.; Lam, D.J.

    1982-01-01

    One aspect of the leachability of actinide-bearing glass which has not been adequately addressed is the effect of radiolysis of the system (glass-water) on the amount of actinides liberated from the glass. In the present study, we have investigated the leaching of plutonium and americium from 76-101 glass samples (containing 2 mole % plutonium) in the presence of a one megaRad/hour gamma-radiation field. The presence of the radiation field was found to increase the leaching rate of both plutonium and americium by a factor of five. Speciation studies of the plutonium in the leachate indicate that the plutonium is present predominantly in the higher oxidation states, Pu(V) and Pu(VI) and that it is significantly associated with colloidal particles. Examination of the glass surfaces with x-ray photoemission spectroscopy, XPS, both before and after leaching was carried out; these studies showed lower surface concentrations of plutonium in the samples of glass leached in the radiation field. 1 figure, 3 tables.

  5. Osteosarcoma induction by plutonium-239, americium-241 and neptunium-237 : the problem of deriving risk estimates for man

    International Nuclear Information System (INIS)

    Spontaneous bone cancer (osteosarcoma) represents only about 0.3% of all human cancers, but is well known to be inducible in humans by internal contamination with radium-226 and radium-224. plutonium-239, americium-241 and neptunium-237 form, or will form, the principal long-lived alpha particle emitting components of high activity waste and burnt-up nuclear fuel elements. These three nuclides deposit extensively in human bone and although, fortunately, no case of a human osteosarcoma induced by any of these nuclides is known, evidence from animal studies suggests that all three are more effective than radium-226 in inducing osteosarcoma. The assumption that the ratio of the risk factors, the number of osteosarcoma expected per 10000 person/animal Gy, for radium-226 and any other bone-seeking alpha-emitter will be independent of animal species has formed the basis of all the important studies of the radiotoxicity of actinide nuclides in experimental animals. The aim of this communication is to review the risk factors which may be calculated from the various animal studies carried out over the last thirty years with plutonium-237, americium-241 and neptunium-237 and to consider the problems which may arise in extrapolating these risk factors to homo sapiens

  6. Precise measurement and analysis of neutron transmission through 232Th

    International Nuclear Information System (INIS)

    Three sets of transmission time spectra through up to eight samples of 232Th have been measured for neutron energies from 6.0 MeV to 0.1 MeV by use of a flight-time technique over 22- and 40-m path lengths, the ORELA pulsed neutron source, and a 1-mm-thick lithium glass detector. The resulting total cross section from 0.1 to 20.0 eV seems to be smaller than that contained in the ENDF/B-V evaluation. Least-squares analysis of the transmissions from 9 to 440 eV using a multilevel Breit-Wigner formalism results in neutron widths consistent with those previously reported. An average radiation width of 25.2 MeV is obtained for 19 low-energy s-wave resonances. 3 figures, 5 tables

  7. Experimental Study on Behavior of Americium in Pyrochemical Process of Nitride Fuel Cycle

    International Nuclear Information System (INIS)

    R and D on the transmutation of long-lived minor actinides (MA) by the accelerator-driven system (ADS) using nitride fuels is underway at JAEA. In regard to reprocessing technology, pyrochemical process has several advantages in case of treating spent fuel with large decay heat and fast neutron emission, and recovering highly enriched N-15. In the pyrochemical reprocessing, plutonium and MA are dissolved in LiCl-KCl eutectic melts and selectively recovered into liquid cadmium (Cd) cathode by molten salt electrorefining. The electrochemical behavior in LiCl-KCl eutectic melts and the subsequent nitride formation behavior of plutonium and MA recovered in liquid Cd cathode are investigated. In this paper, recent results on electrochemical study of americium (Am) on electrolyses of AmN in LiCl-KCl eutectic melts and nitride formation of Am recovered in the liquid Cd cathode are presented. Electrochemical behavior of Am on anodic dissolution of AmN and recovery of Am into a liquid Cd cathode by electrolyses in LiCl-KCl eutectic melts was investigated by transient electrochemical techniques. The formal standard potential of Am(III)/Am(0) obtained with the liquid Cd electrode is more positive than that calculated for the solid metal electrode. The potential shift is considered to be attributed to the lowering of the activity of Am by the formation of the intermetallic compound with Cd. Potentiostatic electrolyses of AmN in LiCl-KCl eutectic melts containing AmCl3 at 773 K were carried out. Nitrogen gas generated by the anodic dissolution of AmN was observed, and the current efficiency was obtained from the ratio of the amount of released nitrogen gas and the passed electric charge to be 20 - 28 %. Am was recovered as Am-Cd alloy in the liquid Cd cathode, in which AmCd6 type phase was identified besides Cd phase. The recovered Am was converted to AmN by the nitridation-distillation combined method, in which the Am-Cd alloy was heated in nitrogen gas stream at 973 K. These

  8. 17 CFR 232.406T - Temporary rule related to Interactive Data Files.

    Science.gov (United States)

    2010-04-01

    ... 17 Commodity and Securities Exchanges 2 2010-04-01 2010-04-01 false Temporary rule related to Interactive Data Files. 232.406T Section 232.406T Commodity and Securities Exchanges SECURITIES AND EXCHANGE COMMISSION REGULATION S-T-GENERAL RULES AND REGULATIONS FOR ELECTRONIC FILINGS Xbrl-Related Documents §...

  9. 48 CFR 52.232-31 - Invitation To Propose Financing Terms.

    Science.gov (United States)

    2010-10-01

    ... 48 Federal Acquisition Regulations System 2 2010-10-01 2010-10-01 false Invitation To Propose Financing Terms. 52.232-31 Section 52.232-31 Federal Acquisition Regulations System FEDERAL ACQUISITION... contractual language describing the contract financing (see FAR 32.202-2 for appropriate definitions of...

  10. 24 CFR 1000.232 - Can an Indian tribe or TDHE amend its IHP?

    Science.gov (United States)

    2010-04-01

    ... its IHP? 1000.232 Section 1000.232 Housing and Urban Development Regulations Relating to Housing and... an Indian tribe or TDHE amend its IHP? Yes. Section 103(c) of NAHASDA specifically provides that a recipient may submit modifications or revisions of its IHP to HUD. Unless the initial IHP...

  11. 42 CFR 414.232 - Special payment rules for transcutaneous electrical nerve stimulators (TENS).

    Science.gov (United States)

    2010-10-01

    ... nerve stimulators (TENS). 414.232 Section 414.232 Public Health CENTERS FOR MEDICARE & MEDICAID SERVICES... Special payment rules for transcutaneous electrical nerve stimulators (TENS). (a) General payment rule. Except as provided in paragraph (b) of this section, payment for TENS is made on a purchase basis...

  12. 49 CFR 232.505 - Pre-revenue service acceptance testing plan.

    Science.gov (United States)

    2010-10-01

    ... 49 Transportation 4 2010-10-01 2010-10-01 false Pre-revenue service acceptance testing plan. 232... § 232.505 Pre-revenue service acceptance testing plan. (a) General; submission of plan. Except as... its system the operating railroad or railroads shall submit a pre-revenue service acceptance...

  13. 48 CFR 52.232-30 - Installment Payments for Commercial Items.

    Science.gov (United States)

    2010-10-01

    ... 48 Federal Acquisition Regulations System 2 2010-10-01 2010-10-01 false Installment Payments for Commercial Items. 52.232-30 Section 52.232-30 Federal Acquisition Regulations System FEDERAL ACQUISITION... requests shall be paid within 30 days of submittal of a proper request for payment. (e) Liquidation...

  14. [Uptake of radionuclides from soil to plant and the discovery of 226Ra, 232Th hyperaccumulator].

    Science.gov (United States)

    Zhang, Zhi-Qiang; Chen, Di-Yun; Song, Gang; Yue, Yu-Mei

    2011-04-01

    11 sorts of plant samples and corresponding soil samples were collected in Conghua and Taishan, Pearl River Delta. The specific activity of 238U, 226Ra, 232Th and 40K of samples were investigated by using HPGe-gamma-ray spectra analysis. The results showed that the average specific activity of 238U, 226Ra, 232Th and 40K in soil samples were 151.8, 146.3, 226.6, 665.5 Bq/kg, which were higher than the average values of China and the world. The concentration of 238U in all sort of plants are very low and most of them are lower than detection limit, while the values of 226Ra, 232Th and 40K were high. The contents of 226Ra and 232Th in Dicranopteris dichotoma were the highest, whose average specific activity is 285.9, 986.2 Bq/kg respectively. The average bioconcentration factors (BFs)of 26Ra, 232Th of Dicranopteris dichotoma were 2.20, 4.23, respectively, the other 10 sort of plants have BFs of 2266Ra, 232Th were in the range of 10(-1)-10(-2). The bioconcentration factors and the translocation factors of 226Ra, 232Th of Dicranopteris dichotoma. were all bigger than 1, so Dicranopteris dichotoma can be defined as hyperaccumulator of 226Ra and 232Th. PMID:21717763

  15. LIBS Spectral Data for a Mixed Actinide Fuel Pellet Containing Uranium, Plutonium, Neptunium and Americium

    Energy Technology Data Exchange (ETDEWEB)

    Judge, Elizabeth J. [Los Alamos National Laboratory; Berg, John M. [Los Alamos National Laboratory; Le, Loan A. [Los Alamos National Laboratory; Lopez, Leon N. [Los Alamos National Laboratory; Barefield, James E. [Los Alamos National Laboratory

    2012-06-18

    Laser-induced breakdown spectroscopy (LIBS) was used to analyze a mixed actinide fuel pellet containing 75% UO{sub 2}/20% PuO{sub 2}/3% AmO{sub 2}/2% NpO{sub 2}. The preliminary data shown here is the first report of LIBS analysis of a mixed actinide fuel pellet, to the authors knowledge. The LIBS spectral data was acquired in a plutonium facility at Los Alamos National Laboratory where the sample was contained within a glove box. The initial installation of the glove box was not intended for complete ultraviolet (UV), visible (VIS) and near infrared (NIR) transmission, therefore the LIBS spectrum is truncated in the UV and NIR regions due to the optical transmission of the window port and filters that were installed. The optical collection of the emission from the LIBS plasma will be optimized in the future. However, the preliminary LIBS data acquired is worth reporting due to the uniqueness of the sample and spectral data. The analysis of several actinides in the presence of each other is an important feature of this analysis since traditional methods must chemically separate uranium, plutonium, neptunium, and americium prior to analysis. Due to the historic nature of the sample fuel pellet analyzed, the provided sample composition of 75% UO{sub 2}/20% PuO{sub 2}/3% AmO{sub 2}/2% NpO{sub 2} cannot be confirm without further analytical processing. Uranium, plutonium, and americium emission lines were abundant and easily assigned while neptunium was more difficult to identify. There may be several reasons for this observation, other than knowing the exact sample composition of the fuel pellet. First, the atomic emission wavelength resources for neptunium are limited and such techniques as hollow cathode discharge lamp have different dynamics than the plasma used in LIBS which results in different emission spectra. Secondly, due to the complex sample of four actinide elements, which all have very dense electronic energy levels, there may be reactions and

  16. Preconcentration of low levels of americium and plutonium from waste waters by synthetic water-soluble metal-binding polymers with ultrafiltration

    International Nuclear Information System (INIS)

    A preconcentration approach to assist in the measurement of low levels of americium and plutonium in waste waters has been developed based on the concept of using water-soluble metal-binding polymers in combination with ultrafiltration. The method has been optimized to give over 90% recovery and accountability from actual waste water. (author)

  17. Theoretical investigation of pressure-induced structural transitions in americium using GGA+U and hybrid density functional theory methods

    DEFF Research Database (Denmark)

    Verma, Ashok K.; Modak, P.; Sharma, Surinder M.;

    2013-01-01

    First-principles calculations have been performed for americium (Am) metal using the generalized gradient approximation + orbital-dependent onsite Coulomb repulsion via Hubbard interaction (GGA+U) and hybrid density functional theory (HYB-DFT) methods to investigate various ground state propertie...

  18. Molecular characteristic and pathogenicity of Indonesian H5N1 clade 2.3.2 viruses

    Directory of Open Access Journals (Sweden)

    Dharmayanti NLPI

    2013-06-01

    Full Text Available The outbreak of disease in late 2012 in Indonesia caused high duck mortality. The agent of the disease was identified as H5N1 clade 2.3.2. The disease caused economic loss to the Indonesian duck farmer. The clade 2.3.2 of H5N1 virus has not previously been identified, so this study was conducted to characterize 4 of H5N1 clade 2.3.2 viruses by DNA sequencing in eight genes segment virus namely HA, NA, NS, M, PB1, PB2, PA and NP. The pathogenicity test of clade 2.3.2 viruses in ducks was compared to clade 2.1.3 viruses which predominat circulating in Indonesia. Results of phylogenetic tree analysis showed that the four of clade 2.3.2 viruses isolated in 2012 was the new introduced virus from abroad. Further analysis showed eight genes were in one group with the clade 2.3.2 viruses, especially those from VietNam and did not belong to Indonesia viruses group. The pathogenicity test in ducks showed that virus H5N1 clade 2.3.2 and clade 2.1.3 have similar clinical symptoms and pathogenicity and cause death in 75% of ducks on days 3-6 after infection.

  19. 48 CFR 52.232-35 - Designation of Office for Government Receipt of Electronic Funds Transfer Information.

    Science.gov (United States)

    2010-10-01

    ... Government Receipt of Electronic Funds Transfer Information. 52.232-35 Section 52.232-35 Federal Acquisition... CONTRACT CLAUSES Text of Provisions and Clauses 52.232-35 Designation of Office for Government Receipt of Electronic Funds Transfer Information. As prescribed in 32.1110(c), insert the following clause:...

  20. 17 CFR 232.313 - Identification of investment company type and series and/or class (or contract).

    Science.gov (United States)

    2010-04-01

    ... company type and series and/or class (or contract). 232.313 Section 232.313 Commodity and Securities Exchanges SECURITIES AND EXCHANGE COMMISSION REGULATION S-T-GENERAL RULES AND REGULATIONS FOR ELECTRONIC FILINGS Preparation of Electronic Submissions § 232.313 Identification of investment company type...

  1. Design of USB 、RS232/RS422 interface convertion circuit%USB、RS232/S422接口转换电路的设计

    Institute of Scientific and Technical Information of China (English)

    黄燕妮; 王少云

    2012-01-01

    由于USB接口正逐步替代传统的RS232接口成为PC机的标准接口,USB接口转换电路的设计就很有必要。采用Silicon公司高集成度的USB—UART桥接器件CP2102,辅以简单的外部电路,实现了RS232/RS422接口与USB接口转换电路的设计。其中在详细介绍CP2102结构和特性的基础上,给出了接口转换的硬件电路图,最后简单介绍了转换器的工作原理。%Due to USB(Universal Serial Bus) interface is gradually replacing the traditional RS232 interface,and becoming the PC standard interface, the conversion circuit of USB,RS232 / RS422 interface is important and necessary. Using Silicon's CP2102 which is highly-integrated USB to UART bridge device, the paper provides USB interface convertion with a simple external circuit. On the basis of introducting the feature and structure of CP2102, the paper gives how to design hardware circuit of USB ,RS232 / RS422 interface conversion and how to use it.

  2. Gamma-spectrometric determination of {sup 232}U in uranium-bearing materials

    Energy Technology Data Exchange (ETDEWEB)

    Zsigrai, Jozsef [European Commission, Joint Research Centre (JRC), Institute for Transuranium Elements (ITU), 76125 Karlsruhe, P.O. Box 2340 (Germany); Nguyen, Tam Cong [Centre for Energy Research of the Hungarian Academy of Sciences (EK), 1525 Budapest 114, P.O. Box 49 (Hungary); Berlizov, Andrey [European Commission, Joint Research Centre (JRC), Institute for Transuranium Elements (ITU), 76125 Karlsruhe, P.O. Box 2340 (Germany)

    2015-09-15

    The {sup 232}U content of various uranium-bearing items was measured using low-background gamma spectrometry. The method is independent of the measurement geometry, sample form and chemical composition. Since {sup 232}U is an artificially produced isotope, it carries information about previous irradiation of the material, which is relevant for nuclear forensics, nuclear safeguards and for nuclear reactor operations. A correlation between the {sup 232}U content and {sup 235}U enrichment of the investigated samples has been established, which is consistent with theoretical predictions. It is also shown how the correlation of the mass ratio {sup 232}U/{sup 235}U vs. {sup 235}U content can be used to distinguish materials contaminated with reprocessed uranium from materials made of reprocessed uranium.

  3. Gamma-spectrometric determination of 232U in uranium-bearing materials

    International Nuclear Information System (INIS)

    The 232U content of various uranium-bearing items was measured using low-background gamma spectrometry. The method is independent of the measurement geometry, sample form and chemical composition. Since 232U is an artificially produced isotope, it carries information about previous irradiation of the material, which is relevant for nuclear forensics, nuclear safeguards and for nuclear reactor operations. A correlation between the 232U content and 235U enrichment of the investigated samples has been established, which is consistent with theoretical predictions. It is also shown how the correlation of the mass ratio 232U/235U vs. 235U content can be used to distinguish materials contaminated with reprocessed uranium from materials made of reprocessed uranium

  4. Gamma-spectrometric determination of 232U in uranium-bearing materials

    CERN Document Server

    Zsigrai, Jozsef; Berlizov, Andriy

    2015-01-01

    The 232U content of various uranium-bearing items was measured using low-background gamma-spectrometry. The method is independent of the measurement geometry, sample form and chemical composition. Since 232U is an artificially produced isotope, it carries information about previous irradiation of the material, which is relevant for nuclear forensics, nuclear safeguards and for nuclear reactor operations. A correlation between the 232U content and 235U enrichment of the investigated samples has been established, which is consistent with theoretical predictions. It is also shown how the correlation of the mass ratio 232U/235U vs. 235U content can be used to distinguish materials contaminated with reprocessed uranium from materials made of reprocessed uranium.

  5. The ID23-2 structural biology microfocus beamline at the ESRF

    Energy Technology Data Exchange (ETDEWEB)

    Flot, David, E-mail: flot@esrf.fr [European Molecular Biology Laboratory, 6 rue Jules Horowitz, BP 181, 38042 Grenoble (France); Mairs, Trevor; Giraud, Thierry; Guijarro, Matias; Lesourd, Marc; Rey, Vicente; Brussel, Denis van; Morawe, Christian; Borel, Christine; Hignette, Olivier; Chavanne, Joel; Nurizzo, Didier; McSweeney, Sean; Mitchell, Edward [European Synchrotron Radiation Facility, 6 rue Jules Horowitz, BP 181, 38043 Grenoble (France)

    2010-01-01

    Beamline ID23-2, the first dedicated and highly automated high-throughput monochromatic macromolecular crystallography microfocus beamline, is described. The first phase of the ESRF beamline ID23 to be constructed was ID23-1, a tunable MAD-capable beamline which opened to users in early 2004. The second phase of the beamline to be constructed is ID23-2, a monochromatic microfocus beamline dedicated to macromolecular crystallography experiments. Beamline ID23-2 makes use of well characterized optical elements: a single-bounce silicon (111) monochromator and two mirrors in Kirkpatrick–Baez geometry to focus the X-ray beam. A major design goal of the ID23-2 beamline is to provide a reliable, easy-to-use and routine microfocus beam. ID23-2 started operation in November 2005, as the first beamline dedicated to microfocus macromolecular crystallography. The beamline has taken the standard automated ESRF macromolecular crystallography environment (both hardware and software), allowing users of ID23-2 to be rapidly familiar with the microfocus environment. This paper describes the beamline design, the special considerations taken into account given the microfocus beam, and summarizes the results of the first years of the beamline operation.

  6. Stability of penta- and hexavalent americium in the solutions of sodium peroxydisulfate and sodium bromate at intensive internal α-irradiation

    International Nuclear Information System (INIS)

    The spectrometric method has been used for studying the dependence of the rates of radiolytic reduction of Am(5) and (6) on the initial concentration of sodium persulfate and bromate, Am(5) and (6), acidity, and the dose rate of inner alpha-irradiation of the solutions. The high dose rates of inner alpha-irradiation of solutions (up to 3.25x1021 eV/lxmin-250Ci/l) have been attained with the aid of curium isotopes. The stability of americium (6) ions towards the action of ionizing radiation in solutions of sodium persulfate and bromate has been shown to be considerable lower than that of americium (5). The chemical difference has been shown in radiolytic behaviour between Am(5) and Am(6) ions in solutions of sodium persulfate and bromate. The equations have been derived showing the dependence of the rates of Am(6) and Am(5) reduction of different variables

  7. Comparative XRPD and XAS study of the impact of the synthesis process on the electronic and structural environments of uranium-americium mixed oxides

    Science.gov (United States)

    Prieur, D.; Lebreton, F.; Martin, P. M.; Caisso, M.; Butzbach, R.; Somers, J.; Delahaye, T.

    2015-10-01

    Uranium-americium mixed oxides are potential compounds to reduce americium inventory in nuclear waste via a partitioning and transmutation strategy. A thorough assessment of the oxygen-to-metal ratio is paramount in such materials as it determines the important underlying electronic structure and phase relations, affecting both thermal conductivity of the material and its interaction with the cladding and coolant. In 2011, various XAS experiments on U1-xAmxO2±δ samples prepared by different synthesis methods have reported contradictory results on the charge distribution of U and Am. This work alleviates this discrepancy. The XAS results confirm that, independently of the synthesis process, the reductive sintering of U1-xAmxO2±δ leads to the formation of similar fluorite solid solution indicating the presence of Am+III and U+V in equimolar proportions.

  8. THE FIRST ISOLATION OF AMERICIUM IN THE FORM OF PURE COMPOUNDS - THE SPECIFIC ALPHA-ACTIVITY AND HALF-LIFE OF Am241

    Energy Technology Data Exchange (ETDEWEB)

    Cunningham, B.B.; Asprey, L.B.

    1950-07-20

    The microgram scale isolation and preparation of pure compounds of americium is described. Data are presented to show that the alpha-half-life of the isotope Am{sup 241} is 490 {+-} 14 years. The absorption spectrum of Am(III) in 1M nitric acid in the range 3500-8000 mu is given. The wave lengths of 10 of the most prominent lines in the copper spark emission spectrum of americium are given to the nearest 0.01 {angstrom}. Evidence is presented to show that the potential for the Am(III)-Am(IV) couple in acid solution is more negative than -2v and that the potential for the Am(II)-Am(III) couple is more positive than +0.9v.

  9. A Density Functional Study of Atomic Hydrogen and Oxygen Chemisorption on the Relaxed (0001) Surface of Double Hexagonal Close Packed Americium

    OpenAIRE

    Dholabhai, P. P.; Atta-Fynn, R.; A.K. Ray

    2009-01-01

    Ab initio total energy calculations within the framework of density functional theory have been performed for atomic hydrogen and oxygen chemisorption on the (0001) surface of double hexagonal packed americium using a full-potential all-electron linearized augmented plane wave plus local orbitals method. Chemisorption energies were optimized with respect to the distance of the adatom from the relaxed surface for three adsorption sites, namely top, bridge, and hollow hcp sites, the adlayer str...

  10. Experimental study of Americium-241 biokinetics in Homarus Gammarus lobster. Analysis of the accumulation and detoxication mechanisms at the sub-cellular level

    International Nuclear Information System (INIS)

    The Americium 241 radioelement accumulation and elimination rate and mechanisms in the lobster organism have been experimentally studied; incorporation and detoxification capacities of each organ are evaluated. The existence of various biological compartments is shown; the major role of the digestive gland in accumulation of the radioelement, its distribution towards the various organs, and its resorption is comprehensively described, with an analysis at the subcellular and molecular levels. 401 p., 65 fig., 43 tab., 428 ref

  11. A new method for the determination of plutonium and americium using high pressure microwave digestion and alpha-spectrometry or ICP-SMS

    International Nuclear Information System (INIS)

    Plutonium and americium are radionuclides particularly difficult to measure in environmental samples because they are a-emitters and therefore necessitate a careful separation before any measurement, either using radiometric methods or ICP-SMS. Recent developments in extraction chromatography resins such as EichromR TRU and TEVA have resolved many of the analytical problems but drawbacks such as low recovery and spectral interferences still occasionally occur. Here, we report on the use of the new EichromR DGA resin in association with TEVA resin and high pressure microwave acid leaching for the sequential determination of plutonium and americium in environmental samples. The method results in average recoveries of 83 ± 15% for plutonium and 73 ± 22% for americium (n = 60), and a less than 10% deviation from reference values of four IAEA reference materials and three samples from intercomparisons exercises. The method is also suitable for measuring 239Pu in water samples at the μBq/l level, if ICP-SMS is used for the measurement. (author)

  12. An experimental study of americium-241 biokinetics in the Lobster Homarus Gammarus. Analysis of the accumulation/storage and detoxification processes at the subcellular level

    International Nuclear Information System (INIS)

    An experimental study of americium-241 kinetics has been conducted in the lobster Homarus gammmarus. The investigations were conducted at all the levels from the whole body to the subcellular and molecular levels. The animals were contaminated by a single or chronic ingestion of 241 Am labelled mussels. Assessments of accumulation, elimination and distribution of the radionuclide were established on organisms kept in the laboratory; they made it possible to demonstrate the importance of the digestive gland in the radionuclide transfer pathways. The preliminary results led to structural then ultrastructural investigations of the digestive gland in association with radioautographic studies and cellular extractions methods. Four cellular types were demonstrated, only two of them being implied in the radionuclide retention, the former being responsible for americium intake and the latter for its long-term retention. By means of biochemical techniques, subcellular accumulation was studied and the organelles implied in the nuclide retention were specified. Finally, a method of cellular nuclei dissociation was developed; it made it possible to analyse the molecular nature of americium ligands and to demonstrate the function of the protein nuclear matrix in the nuclide retention

  13. Comparative XRPD and XAS study of the impact of the synthesis process on the electronic and structural environments of uranium–americium mixed oxides

    Energy Technology Data Exchange (ETDEWEB)

    Prieur, D., E-mail: dam.prieur@gmail.com [European Commission, Joint Research Centre, Institute for Transuranium Elements, P.O. Box 2340, D-76125 Karlsruhe (Germany); Lebreton, F. [CEA, DEN, DTEC/SDTC/LEMA, 30207 Bagnols-sur-Cèze cedex (France); Martin, P.M. [CEA, DEN, DEC/SESC/LLCC, 13108 Saint-Paul-Lez-Durance cedex (France); Caisso, M. [CEA, DEN, DTEC/SDTC/LEMA, 30207 Bagnols-sur-Cèze cedex (France); Butzbach, R. [Helmholtz Zentrum Dresden Rossendorf (HZDR), Institute of Radiochemistry, P.O. Box 10119, 01314 Dresden (Germany); Somers, J. [European Commission, Joint Research Centre, Institute for Transuranium Elements, P.O. Box 2340, D-76125 Karlsruhe (Germany); Delahaye, T. [CEA, DEN, DTEC/SDTC/LEMA, 30207 Bagnols-sur-Cèze cedex (France)

    2015-10-15

    Uranium–americium mixed oxides are potential compounds to reduce americium inventory in nuclear waste via a partitioning and transmutation strategy. A thorough assessment of the oxygen-to-metal ratio is paramount in such materials as it determines the important underlying electronic structure and phase relations, affecting both thermal conductivity of the material and its interaction with the cladding and coolant. In 2011, various XAS experiments on U{sub 1−x}Am{sub x}O{sub 2±δ} samples prepared by different synthesis methods have reported contradictory results on the charge distribution of U and Am. This work alleviates this discrepancy. The XAS results confirm that, independently of the synthesis process, the reductive sintering of U{sub 1−x}Am{sub x}O{sub 2±δ} leads to the formation of similar fluorite solid solution indicating the presence of Am{sup +III} and U{sup +V} in equimolar proportions. - Graphical abstract: Formation of (U{sup IV/V},Am{sup III})O{sup 2} solid solution by sol–gel and by powder metallurgy. - Highlights: • Uranium–americium mixed oxides were synthesized by sol–gel and powder metallurgy. • Fluorite solid solutions with similar local environment have been obtained. • U{sup V} and Am{sup III} are formed in equimolar proportions.

  14. Use of radioanalytical methods for determination of uranium, neptunium, plutonium, americium and curium isotopes in radioactive wastes

    International Nuclear Information System (INIS)

    Activated charcoal is a common type of radioactive waste that contains high concentrations of fission and activation products. The management of this waste includes its characterization aiming the determination and quantification of the specific radionuclides including those known as Difficult-to-Measure Radionuclides (RDM). The analysis of the RDM's generally involves complex radiochemical analysis for purification and separation of the radionuclides, which are expensive and time-consuming. The objective of this work was to define a methodology for sequential analysis of the isotopes of uranium, neptunium, plutonium, americium and curium present in a type of radioactive waste, evaluating chemical yield, analysis of time spent, amount of secondary waste generated and cost. Three methodologies were compared and validated that employ ion exchange (TI + EC), extraction chromatography (EC) and extraction with polymers (ECP). The waste chosen was the activated charcoal from the purification system of primary circuit water cooling the reactor IEA-R1. The charcoal samples were dissolved by acid digestion followed by purification and separation of isotopes with ion exchange resins, extraction and chromatographic extraction polymers. Isotopes were analyzed on an alpha spectrometer, equipped with surface barrier detectors. The chemical yields were satisfactory for the methods TI + EC and EC. ECP method was comparable with those methods only for uranium. Statistical analysis as well the analysis of time spent, amount of secondary waste generated and cost revealed that EC method is the most effective for identifying and quantifying U, Np, Pu, Am and Cm present in charcoal. (author)

  15. Intramolecular sensitization of americium luminescence in solution: shining light on short-lived forbidden 5f transitions.

    Science.gov (United States)

    Sturzbecher-Hoehne, M; Yang, P; D'Aléo, A; Abergel, R J

    2016-06-14

    The photophysical properties and solution thermodynamics of water soluble trivalent americium (Am(III)) complexes formed with multidentate chromophore-bearing ligands, 3,4,3-LI(1,2-HOPO), Enterobactin, and 5-LIO(Me-3,2-HOPO), were investigated. The three chelators were shown to act as antenna chromophores for Am(III), generating sensitized luminescence emission from the metal upon complexation, with very short lifetimes ranging from 33 to 42 ns and low luminescence quantum yields (10(-3) to 10(-2)%), characteristic of Near Infra-Red emitters in similar systems. The specific emission peak of Am(III) assigned to the (5)D1 → (7)F1 f-f transition was exploited to characterize the high proton-independent stability of the complex formed with the most efficient sensitizer 3,4,3-LI(1,2-HOPO), with a log β110 = 20.4 ± 0.2 value. In addition, the optical and solution thermodynamic features of these Am(III) complexes, combined with density functional theory calculations, were used to probe the influence of electronic structure on coordination properties across the f-element series and to gain insight into ligand field effects.

  16. Nano-cerium vanadate: a novel inorganic ion exchanger for removal of americium and uranium from simulated aqueous nuclear waste.

    Science.gov (United States)

    Banerjee, Chayan; Dudwadkar, Nilesh; Tripathi, Subhash Chandra; Gandhi, Pritam Maniklal; Grover, Vinita; Kaushik, Chetan Prakash; Tyagi, Avesh Kumar

    2014-09-15

    Cerium vanadate nanopowders were synthesized by a facile low temperature co-precipitation method. The product was characterized by X-ray diffraction and transmission electron microscopy and found to consist of ∼25 nm spherical nanoparticles. The efficiency of these nanopowders for uptake of alpha-emitting radionuclides (233)U (4.82 MeV α) and (241)Am (5.49 MeV α, 60 keV γ) has been investigated. Thermodynamically and kinetically favorable uptake of these radionuclides resulted in their complete removal within 3h from aqueous acidic feed solutions. The uptake capacity was observed to increase with increase in pH as the zeta potential value decreased with the increase in pH but effect of ionic strength was insignificant. Little influence of the ions like Sr(2+), Ru(3+), Fe(3+), etc., in the uptake process indicated CeVO4 nanopowders to be amenable for practical applications. The isotherms indicated predominant uptake of the radioactive metal ions in the solid phase of the exchanger at lower feed concentrations and linear Kielland plots with positive slopes indicated favorable exchange of the metal ions with the nanopowder. Performance comparison with the other sorbents reported indicated excellent potential of nano-cerium vanadate for removing americium and uranium from large volumes of aqueous acidic solutions.

  17. Distribution of plutonium, americium, and several rare earth fission product elements between liquid cadmium and LiCl-KCl eutectic

    International Nuclear Information System (INIS)

    Separation factors were measured that describe the partition between molten cadmium and molten LiCl-KCl eutectic of plutonium, americium, praseodymium, neodymium, cerium, lanthanum, gadolinium, dysprosium, and yttrium. The temperature range was 753-788 K, and the range of concentrations was that allowed by the sensitivity of the chemical analysis methods. Mean separation factors were derived for Am-Pu, Nd-Am, Nd-Pu, Nd-Pr, Gd-La, Dy-La, La-Ce, La-Nd, Y-La, and Y-Nd. Where previously published data were available, agreement was good. For convenience, the following series of separation factors relative to plutonium was derived by combining the measured separation factors: Pu, 1.00 (basis); Am, 1.54; Pr, 22.0; Nd, 23.4; Ce, 26; La, 70; Gd, 77; Dy, 270; Y, 3000. These data are used in calculating the distribution of the actinide and rare earth elements in the prochemical reprocessing of spent fuel from the Integral Fast Reactor. (orig.)

  18. Evaluation of synthetic water-soluble metal-binding polymers with ultrafiltration for selective concentration of americium and plutonium

    International Nuclear Information System (INIS)

    Routine counting methods and ICP-MS are unable to directly measure the new US Department of Energy (DOE) regulatory level for discharge waters containing alpha-emitting radionuclides of 30 pCi/L total alpha or the 0.05 pCi/L regulatory level for Pu or Am activity required for surface waters at the Rocky Flats site by the State of Colorado. This inability indicates the need to develop rapid, reliable, and robust analytical techniques for measuring actinide metal ions, particularly americium and plutonium. Selective separation or preconcentration techniques would aid in this effort. Water-soluble metal-binding polymers in combination with ultrafiltration are shown to be an effective method for selectively removing dilute actinide ions from acidic solutions of high ionic strength. The actinide-binding properties of commercially available water-soluble polymers and several polymers which have been reported in the literature were evaluated. The functional groups incorporated in the polymers were pyrrolidone, amine, oxime, and carboxylic, phosphonic, or sulfonic acid. The polymer containing phosphonic acid groups gave the best results with high distribution coefficients and concentration factors for 241Am(III) and 238Pu(III)/(IV) at pH 4 to 6 and ionic strengths of 0.1 to 4

  19. Characteristics of plutonium and americium contamination at the former U.K. atomic weapons test ranges at Maralinga and Emu

    International Nuclear Information System (INIS)

    Physico-chemical studies on environmental plutonium are described, which provide data integral to an assessment of dose for the inhalation of artificial actinides by Australian Aborigines living a semi-traditional lifestyle at Maralinga and Emu, sites of U.K. atomic weapons tests between 1953 and 1963. The most significant area, from a radiological perspective, is the area contaminated by plutonium in a series of ''one point'' safety trials in which large quantities of plutonium were dispersed explosively at a location known as Taranaki. The activity distribution of plutonium and americium with particle size is quite different from the mass distribution, as a considerably higher proportion of the activity is contained in the finer (inhalable) fraction than of the mass. Except in areas which were disturbed through ploughing during a cleanup in 1967, most the activity remains in the top 1 cm of the surface. Much of the activity is in particulate form, even at distances > 20 km from the firing sites, and discrete particles have been located even at distances beyond 100 km. Data are presented which permit the assessment of annual committed doses through the inhalation pathway, for Aborigines living a semi-traditional lifestyle in the areas affected by the Taranaki firings in particular. (author)

  20. Irradiation studies of 231Pa in DHRUVA reactor for preparation of 232U

    International Nuclear Information System (INIS)

    In this paper, identification of the potential source of 231Pa, various stages of its recovery and the sample of 231Pa supplied for trial irradiation are described. For producing 232U, irradiation work is proposed in different stages of irradiation. Various trial irradiations and its results are discussed in this paper along with their specific objectives. A computational estimation of conversion efficiency of 231Pa (∼ 10μg) to 232U in DHRUVA reactor, was carried out. The computational result predicted the conversion efficiency and the results of γ-spectroscopy based analysis of the second trial sample matched well. A first level calculation was also carried out to estimate the tolerable quantity of 232Th to keep the concentration of 233U below 5% in the 232U sample. The radioactivity due to the presence of various impurities present in the sample, during the high fluence irradiation, is being estimated. The feasibility of production of the 232U isotope in DHRUVA reactor has thus been established. (author)

  1. Calculation of fusion time scales in 11B + 237Np, 12C + 232Th and 16O + 232Th reactions in a dynamical trajectory model

    International Nuclear Information System (INIS)

    There are several theoretical models which treat the fusion process and energy dissipation in heavy ion collision in terms of a fluctuating force represented by the coupling between macroscopic and intrinsic degrees of freedom. One such dynamical model has been developed by Feldmeier (1987), where the properties of the dissipative force are determined from a microscopic picture of particle exchange between two nuclei. The macroscopic shapes of the nuclear system are represented by axially symmetric configuration with sharp surfaces. We have used the above model to calculate the fusion time scales for the systems 11B + 237Np, 12C +232Th and 16O + 232Th at 77, 86 and 104 MeV bombarding energies to examine the effect of mass asymmetry in fusion dynamics. (author). 2 figs

  2. CSER 94-013: Classification and access to PFP 232-Z Incinerator Facility and limits on characterization and disassembly activities in 232-Z burning hood

    International Nuclear Information System (INIS)

    This CSER justifies the Limited Control Facility designation for the closed Burning Hood in the PFP 232-Z Incinerator Facility. If the Burning Hood is opened to characterize the plutonium distribution and geometric integrity of the internals or for disassembly of the internals, then the more rigorous Fissionable Material Facility classification is required. Two sets of requirements apply for personnel access, criticality firefighting category for water use, and fissile material movement for the two states of the Burning Hood. The parameters used in the criticality analysis are listed to establish the limits under which this CSER is valid. Determination that the Burning Hood fissile material, moderation, or internal arrangements are outside these limits requires reevaluation of these parameter values and activities at the 232-Z Incinerator Facility. When the Burning Hood is open, water entry is to be prevented by two physical barriers for each water source

  3. Reformation practice of S232 SUCKER sizing machine%S232型祖克浆纱机的改造实践

    Institute of Scientific and Technical Information of China (English)

    刘安君; 窦海萍

    2009-01-01

    为解决祖克S232型浆纱机织轴卷绕故障率高、烘燥温度不稳定、压浆力调节装置失控、经轴退绕张力不稳定的问题,进行了技术改造.通过采用多单元技术对织轴卷绕装置进行了两单元改造,对温控系统、压浆力凋节装置以及经轴退绕装置采用了可编程PLC控制技术,改造后提高了祖克S232型浆纱机的自动化程度,降低了设备故障率,提高了浆纱质量.

  4. Production of 232U from irradiation of standard and thorium-based fuels in PWR reactors

    International Nuclear Information System (INIS)

    The production of small quantities of 232U can induce radiation protection issues in the back end of the fuel cycle, particularly for thorium-based fuels. This is due to its relatively short half life (69 years) and the emission of a high energy gamma ray of 2.6 MeV at the end of its decay chain. With the depletion code MURE, we determine the different reactions pathways, and their proportions, leading to the synthesis of 232U in UO2 and (Th,Pu)O2 fuels irradiated in a PWR. Moreover, the impact, on the 232U production, of cycle times such as time separating the fabrication of the fuel and its irradiation as well as influence of the fissile content has been investigated for UO2 fuel. The impact of the thorium ore provenance and of the plutonium quality has been studied for the (Th,Pu)O2 case. (author)

  5. NT-proBNP on Cobas h 232 in point-of-care testing

    DEFF Research Database (Denmark)

    Gils, Charlotte; Ramanathan, R.; Breindahl, T.;

    2015-01-01

    Background. NT-proBNP may be useful for ruling out heart failure in primary health care. In this study we examined the analytical quality of NT-proBNP in primary health care on the Cobas h 232 point-of-care instrument compared with measurements performed in a hospital laboratory. Materials...... and methods. Blood samples requested for NT-proBNP were collected in primary health care (n = 95) and in a hospital laboratory (n = 107). NT-proBNP was measured on-site on Cobas h 232 instruments both in primary health care centres and at the hospital laboratory and all samples were also analyzed...... with a comparison method at the hospital. Precision, trueness, accuracy, and lot-variation were determined at different concentration levels and evaluated according to acceptance criteria. Furthermore user-friendliness was assessed by questionnaires. Results. For Cobas h 232 repeatability CV was 8...

  6. The novel nootropic compound DM232 (UNIFIRAM) ameliorates memory impairment in mice and rats

    OpenAIRE

    Carla Ghelardini; Nicoletta Galeotti; Fulvio Gualtieri; Dina Manetti; Corrado Bucherelli; Elisabetta Baldi; Alessandro Bartolini

    2002-01-01

    The favorable pharmacological profile exhibited by piracetam stimulated the synthesis of related compounds potentially endowed with a higher nootropic potency. The antiamnesic and procognitive activity of DM232 (unifiram), a new compound structurally related to piracetam, was investigated. Mouse passive avoidance and rat Morris water maze and Social learning tests were employed. DM232 (0.001–1 mg/kg i.p. – 0.01–0.1 1mg/kg p.o.) prevented amnesia induced by scopolamine (1.5 mg/kg i.p.), mecamy...

  7. The role of natural organic matter in the migration behaviour of americium in the Boom Clay - Part 1: migration experiments

    International Nuclear Information System (INIS)

    Full text of publication follows: In demonstrating the suitability of Boom Clay as reference site for studying the disposal of radioactive waste, the role of the relatively high amount of Natural Organic Matter (NOM) present in the Boom Clay on the mobility of critical radionuclides needs to be investigated thoroughly. It is generally accepted that trivalent actinides and lanthanides form strong complexes with humic substances. Complexation of these trivalent radionuclides with NOM present in the Boom Clay may therefore have two opposite effects. If complexed by the aqueous phase NOM (the mobile NOM), the radionuclide transport will be governed by the mobility of these dissolved radionuclide- NOM species. If complexed by the solid phase NOM (the immobile NOM) the migration will be retarded. One of the aims of the EC projects TRANCOM-Clay and TRANCOM-II was to investigate the role of mobile NOM as radionuclide carrier in order to develop a conceptual model for inclusion in a performance assessment (PA) model. The migration behaviour of Americium (used as an analogue for the critical radionuclide Pu) was investigated by complexing 241Am with radiolabelled (14C-labelled) NOM before passing through undisturbed Boom Clay cores contained in columns. The use of two different radionuclides, allows the migration behaviour of both the NOM and the Am to be followed. The results of the migration experiments showed that the Am-NOM complexes dissociated when they came into contact with Boom Clay and that the bulk of Am became immobilised (either as Am complexed to immobile NOM or sorbed to the mineral phase). Only a small percentage of the complex persisted as 'stabilised' Am-OM complex which exhibited slow dissociation kinetics upon moving through the Boom Clay. When the applied radionuclide source also contains Am in the form of an inorganic solid phase (when Am is applied above the solubility limit), a continuous source of Am exists to form 'temporarily stabilised' Am

  8. Experimental study of Americium-241 biokinetics in Homarus Gammarus lobster. Analysis of the accumulation and detoxication mechanisms at the sub-cellular level; Etude experimentale des biocinetiques de l`americium-241 chez le homard homarus gammarus. Analyse des mecanismes d`accumulation et de detoxication au niveau subcellulaire

    Energy Technology Data Exchange (ETDEWEB)

    Paquet, F.

    1991-12-01

    The Americium 241 radioelement accumulation and elimination rate and mechanisms in the lobster organism have been experimentally studied; incorporation and detoxification capacities of each organ are evaluated. The existence of various biological compartments is shown; the major role of the digestive gland in accumulation of the radioelement, its distribution towards the various organs, and its resorption is comprehensively described, with an analysis at the subcellular and molecular levels. 401 p., 65 fig., 43 tab., 428 ref.

  9. Nano-cerium vanadate: A novel inorganic ion exchanger for removal of americium and uranium from simulated aqueous nuclear waste

    Energy Technology Data Exchange (ETDEWEB)

    Banerjee, Chayan; Dudwadkar, Nilesh [Fuel Reprocessing Division, Bhabha Atomic Research Centre, Mumbai 400085 (India); Tripathi, Subhash Chandra, E-mail: sctri001@gmail.com [Fuel Reprocessing Division, Bhabha Atomic Research Centre, Mumbai 400085 (India); Gandhi, Pritam Maniklal [Fuel Reprocessing Division, Bhabha Atomic Research Centre, Mumbai 400085 (India); Grover, Vinita [Waste Management Division, Bhabha Atomic Research Centre, Mumbai 400085 (India); Kaushik, Chetan Prakash [Chemistry Division, Bhabha Atomic Research Centre, Mumbai 400085 (India); Tyagi, Avesh Kumar, E-mail: aktyagi@barc.gov.in [Waste Management Division, Bhabha Atomic Research Centre, Mumbai 400085 (India)

    2014-09-15

    Highlights: • Template free, low temperature synthesis of CeVO{sub 4} nanopowders. • Thermodynamically and kinetically favourable uptake of Am(III) and U(VI) exhibited. • K{sub d} and ΔG° values for Am(III) and U(VI) uptake in pH 1–6 are reported. • Interdiffusion coefficients and zeta potential values in pH 1–6 are reported. • Possible application in low level aqueous nuclear waste remediation. - Abstract: Cerium vanadate nanopowders were synthesized by a facile low temperature co-precipitation method. The product was characterized by X-ray diffraction and transmission electron microscopy and found to consist of ∼25 nm spherical nanoparticles. The efficiency of these nanopowders for uptake of alpha-emitting radionuclides {sup 233}U (4.82 MeV α) and {sup 241}Am (5.49 MeV α, 60 keV γ) has been investigated. Thermodynamically and kinetically favorable uptake of these radionuclides resulted in their complete removal within 3 h from aqueous acidic feed solutions. The uptake capacity was observed to increase with increase in pH as the zeta potential value decreased with the increase in pH but effect of ionic strength was insignificant. Little influence of the ions like Sr{sup 2+}, Ru{sup 3+}, Fe{sup 3+}, etc., in the uptake process indicated CeVO{sub 4} nanopowders to be amenable for practical applications. The isotherms indicated predominant uptake of the radioactive metal ions in the solid phase of the exchanger at lower feed concentrations and linear Kielland plots with positive slopes indicated favorable exchange of the metal ions with the nanopowder. Performance comparison with the other sorbents reported indicated excellent potential of nano-cerium vanadate for removing americium and uranium from large volumes of aqueous acidic solutions.

  10. Plutonium, americium and radiocaesium in the marine environment close to the Vandellos I nuclear power plant before decommissioning

    International Nuclear Information System (INIS)

    The Vandellos nuclear power plant (NPP), releasing low-level radioactive liquid waste to the Mediterranean Sea, is the first to be decommissioned in Spain, after an incident which occurred in 1989. The presence, distribution and uptake of various artificial radionuclides (radiocaesium, plutonium and americium) in the environment close to the plant were studied in seawater, bottom sediments and biota, including Posidonia oceanica, fish, crustaceans and molluscs. Seawater, sediments and Posidonia oceanica showed enhanced levels in the close vicinity of the NPP, although the effect was restricted to its near environment. Maximum concentrations in seawater were 11.6±0.5 Bq m-3 and 16.9±1.2 mBq m-3 for 137Cs and 239,240Pu, respectively. When sediment concentrations were normalized to excess 210Pb, they showed both the short-distance transport of artificial radionuclides from the Vandellos plant and the long-distance transport of 137Cs from the Asco NPP. Posidonia oceanica showed the presence of various gamma-emitters attributed to the impact of the Chernobyl accident, on which the effect of the NPP was superimposed. Seawater, sediment and Posidonia oceanica collected near the plant also showed an enhancement of the plutonium isotopic ratio above the fallout value. The uptake of these radionuclides by marine organisms was detectable but limited. Pelagic fish showed relatively higher 137Cs concentrations and only in the case of demersal fish was the plutonium isotopic ratio increased. The reported levels constitute a set of baseline values against which the impact of the decommissioning operations of the Vandellos I NPP can be studied

  11. Molten salt extraction (MSE) of americium from plutonium metal in CaCl2-KCl-PuCl3 and CaCl2-PuCl3 salt systems

    International Nuclear Information System (INIS)

    Molten salt extraction (MSE) of americium-241 from reactor-grade plutonium has been developed using plutonium trichloride salt in stationary furnaces. Batch runs with oxidized and oxide-free metal have been conducted at temperature ranges between 750 and 945C, and plutonium trichloride concentrations from one to one hundred mole percent. Salt-to-metal ratios of 0.10, 0.15, and 0 30 were examined. The solvent salt was either eutectic 74 mole percent CaCl2 endash 26 mole percent KCl or pure CaCl2. Evidence of trivalent product americium, and effects of temperature, salt-to-metal ratio, and oxide contamination on the americium extraction efficiency are given. 24 refs, 20 figs, 13 tabs

  12. Transfer across the human gut of environmental plutonium, americium, cobalt, caesium and technetium: studies with cockles (Cerastoderma edule) from the Irish Sea.

    Science.gov (United States)

    Hunt, G J

    1998-06-01

    Our previous studies have indicated lower values of the gut transfer factor ('f1 values') for plutonium and americium in winkles (Littorina littorea) than adopted by ICRP. The present study was undertaken primarily to investigate whether this observation extends to other species. Samples of cockles (Carastoderma edule) from Ravenglass, Cumbria were eaten by volunteers who provided 24 h samples of urine and faeces. Urine samples indicated f1 values for cockles which were higher than for winkles; for plutonium these ranged overall up to 7 x 10(-4) with an arithmetic mean in the range (2-3) x 10(-4), and for americium up to 2.6 x 10(-4) with an arithmetic mean of 1.2 x 10(-4). Limited data based on volunteers eating cockles from the Solway suggest that f1 values for americium may be greater at distance from Sellafield. The measured values compare with 5 x 10(-4) used by the ICRP for environmental forms of both elements, which would appear to provide adequate protection when calculating doses from Cumbrian cockles. Data for other nuclides were obtained by analysing faecal samples from the volunteers who ate the Ravenglass cockles. Cobalt-60 showed an f1 value in the region of 0.2, twice the value currently used by ICRP. For 137Cs, variabilities were indicated in the range 0.08 to 0.43, within the ICRP value of f1 = 1.0. Technetium-99 gave f1 values up to about 0.6, in reasonable conformity with the ICRP value of 0.5.

  13. Transfer across the human gut of environmental plutonium, americium, cobalt, caesium and technetium: studies with cockles (Cerastoderma edule) from the Irish Sea

    Energy Technology Data Exchange (ETDEWEB)

    Hunt, G.J. [CEFAS Laboratory, Lowestoft, Suffolk NR33 0HT (United Kingdom)

    1998-06-01

    Our previous studies have indicated lower values of the gut transfer factor ('f{sub L} values') for plutonium and americium in winkles (Littorina littorea) than adopted by ICRP. The present study was undertaken primarily to investigate whether this observation extends to other species. Samples of cockles (Cerastoderma edule) from Ravenglass, Cumbria were eaten by volunteers who provided 24 samples of urine and faeces. Urine samples indicated f{sub L} values for cockles which were higher than for winkles; for plutonium these ranged overall up to 7x10{sup -4} with an arithmetic mean in the range (2-3)x10{sup -4}, and for americium up to 2.6x10{sup -4} with an arithmetic mean of 1.2x10{sup -4}. Limited data based on volunteers eating cockles from the Solway suggest that f{sub L} values for americium may be greater at distance from Sellafield. The measured values compare with 5x10{sup -4} used by the ICRP for environmental forms of both elements, which would appear to provide adequate protection when calculating doses from Cumbrian cockles. Data for other nuclides were obtained by analysing faecal samples from the volunteers who ate the Ravenglass cockles. Cobalt-60 showed an f{sub L} value in the region of 0.2, twice the value currently used by ICRP. For {sup 137}Cs, variabilities were indicated in the range 0.08 to 0.43, within the ICRP value of f{sub L}=1.0. Technetium-99 gave f{sub L} values up to about 0.6, in reasonable conformity with the ICRP value of 0.5. (author)

  14. Determination by gamma-ray spectrometry of the plutonium and americium content of the Pu/Am separation scraps. Application to molten salts; Determination par spectrometrie gamma de la teneur en plutonium et en americium de produits issus de separation Pu/Am. Application aux bains de sels

    Energy Technology Data Exchange (ETDEWEB)

    Godot, A. [CEA Valduc, Dept. de Traitement des Materiaux Nucleaires, 21 - Is-sur-Tille (France); Perot, B. [CEA Cadarache, Dept. de Technologie Nucleaire, Service de Modelisation des Transferts et Mesures Nucleaires, 13 - Saint-Paul-lez-Durance (France)

    2005-07-01

    Within the framework of plutonium recycling operations in CEA Valduc (France), americium is extracted from molten plutonium metal into a molten salt during an electrolysis process. The scraps (spent salt, cathode, and crucible) contain extracted americium and a part of plutonium. Nuclear material management requires a very accurate determination of the plutonium content. Gamma-ray spectroscopy is performed on Molten Salt Extraction (MSE) scraps located inside the glove box, in order to assess the plutonium and americium contents. The measurement accuracy is influenced by the device geometry, nuclear instrumentation, screens located between the sample and the detector, counting statistics and matrix attenuation, self-absorption within the spent salt being very important. The purpose of this study is to validate the 'infinite energy extrapolation' method employed to correct for self-attenuation, and to detect any potential bias. We present a numerical study performed with the MCNP computer code to identify the most influential parameters and some suggestions to improve the measurement accuracy. A final uncertainty of approximately 40% is achieved on the plutonium mass. (authors)

  15. An experimental study of americium-241 biokinetics in the Lobster Homarus Gammarus. Analysis of the accumulation/storage and detoxification processes at the subcellular level; Etude experimentale des biocinetiques de l`americium-241 chez le homard homarus gammarus. Analyse des mecanismes d`accumulation et de detoxication au niveau subcellulaire

    Energy Technology Data Exchange (ETDEWEB)

    Paquet, F.

    1993-01-01

    An experimental study of americium-241 kinetics has been conducted in the lobster Homarus gammmarus. The investigations were conducted at all the levels from the whole body to the subcellular and molecular levels. The animals were contaminated by a single or chronic ingestion of {sup 241} Am labelled mussels. Assessments of accumulation, elimination and distribution of the radionuclide were established on organisms kept in the laboratory; they made it possible to demonstrate the importance of the digestive gland in the radionuclide transfer pathways. The preliminary results led to structural then ultrastructural investigations of the digestive gland in association with radioautographic studies and cellular extractions methods. Four cellular types were demonstrated, only two of them being implied in the radionuclide retention, the former being responsible for americium intake and the latter for its long-term retention. By means of biochemical techniques, subcellular accumulation was studied and the organelles implied in the nuclide retention were specified. Finally, a method of cellular nuclei dissociation was developed; it made it possible to analyse the molecular nature of americium ligands and to demonstrate the function of the protein nuclear matrix in the nuclide retention.

  16. Dissertation on the computer-based exploitation of a coincidence multi parametric recording. Application to the study of the disintegration scheme of Americium 241

    International Nuclear Information System (INIS)

    After having presented the meaning of disintegration scheme (alpha and gamma emissions, internal conversion, mean lifetime), the author highlights the benefits of the use of multi-parametric chain for the recording of correlated parameters, and of the use of a computer for the analysis of bi-parametric information based on contour lines. Using the example of Americium 241, the author shows how these information are obtained (alpha and gamma spectrometry, time measurement), how they are chosen, coded, analysed and stored, and then processed by contour lines

  17. 7 CFR 1951.232 - Water and waste disposal systems which have become part of an urban area.

    Science.gov (United States)

    2010-01-01

    ... 7 Agriculture 14 2010-01-01 2009-01-01 true Water and waste disposal systems which have become part of an urban area. 1951.232 Section 1951.232 Agriculture Regulations of the Department of Agriculture (Continued) RURAL HOUSING SERVICE, RURAL BUSINESS-COOPERATIVE SERVICE, RURAL UTILITIES...

  18. 8 CFR 232.2 - Examination in the United States of alien applicants for benefits under the immigration laws and...

    Science.gov (United States)

    2010-01-01

    ... with 42 CFR part 34 and any additional instructions and guidelines as may be considered necessary by... applicants for benefits under the immigration laws and other aliens. 232.2 Section 232.2 Aliens and Nationality DEPARTMENT OF HOMELAND SECURITY IMMIGRATION REGULATIONS DETENTION OF ALIENS FOR PHYSICAL...

  19. 40 CFR 436.232 - Effluent limitations guidelines representing the degree of effluent reduction attainable by the...

    Science.gov (United States)

    2010-07-01

    ... 40 Protection of Environment 29 2010-07-01 2010-07-01 false Effluent limitations guidelines... technology currently available. 436.232 Section 436.232 Protection of Environment ENVIRONMENTAL PROTECTION AGENCY (CONTINUED) EFFLUENT GUIDELINES AND STANDARDS MINERAL MINING AND PROCESSING POINT SOURCE...

  20. 40 CFR 408.232 - Effluent limitations guidelines representing the degree of effluent reduction attainable by the...

    Science.gov (United States)

    2010-07-01

    ... 40 Protection of Environment 28 2010-07-01 2010-07-01 true Effluent limitations guidelines representing the degree of effluent reduction attainable by the application of the best practicable control technology currently available. 408.232 Section 408.232 Protection of Environment ENVIRONMENTAL...

  1. 48 CFR 3452.232-70 - Prohibition against the use of ED funds to influence legislation or appropriations.

    Science.gov (United States)

    2010-10-01

    ... use of ED funds to influence legislation or appropriations. 3452.232-70 Section 3452.232-70 Federal... funds to influence legislation or appropriations. The following clause is to be used in accordance with 3432.770: Prohibition Against the Use of ED Funds To Influence Legislation or Appropriations (APR...

  2. 17 CFR 232.104 - Unofficial PDF copies included in an electronic submission.

    Science.gov (United States)

    2010-04-01

    ... 17 Commodity and Securities Exchanges 2 2010-04-01 2010-04-01 false Unofficial PDF copies included... Filing Requirements § 232.104 Unofficial PDF copies included in an electronic submission. (a) An... (§ 249.101 of this chapter) or a Form D (§ 239.500 of this chapter), may include one unofficial PDF...

  3. D2.3.2 Evaluation results of the LinkedUp VIDI competition

    NARCIS (Netherlands)

    Drachsler, Hendrik; Stoyanov, Slavi; Herder, Eelco; Marieke, Guy; Maren, Scheffel

    2014-01-01

    This document D2.3.2 is the second report of Task 2.4 - Evaluation of challenge submissions. Task 2.4 is about the actual assessment of the participating projects within the LinkedUp Veni, Vidi and Vici competition on the basis of the LinkedUp Evaluation Framework (D2.2.1). The main objective of Tas

  4. Photo fission cross-section of 232Th, 238U and 237Np

    International Nuclear Information System (INIS)

    In the present work, photo fission cross-section of 232Th, 238U and 237Np evaluated with the help of fission fragment angular distribution measurements by using Bremsstrahlung radiation from 7.4 MeV to 9.0 MeV have been carried out by employing high efficiency SSNTD technique

  5. Investigation of the (232)Th Nucleus Excitations at the FEL {gamma} - Nucleus Colliders

    CERN Document Server

    Koru, H; Sultansoy, S F; Sarer, B

    2001-01-01

    The physics search potential of the FEL {gamma} - Nucleus colliders is analysed using excitations of the (232)Th nucleus. It is shown that, due to the monochromacity of FEL {gamma} beam and high statistics, proposed colliders will play an important role in the field of "traditional" nuclear physics.

  6. 17 CFR 232.402 - Liability for XBRL-Related Documents.

    Science.gov (United States)

    2010-04-01

    ... 17 Commodity and Securities Exchanges 2 2010-04-01 2010-04-01 false Liability for XBRL-Related... REGULATION S-T-GENERAL RULES AND REGULATIONS FOR ELECTRONIC FILINGS Xbrl-Related Documents § 232.402 Liability for XBRL-Related Documents. (a) Not deemed filed for liability purposes. XBRL-Related...

  7. 20 CFR 408.232 - When do you lose your foreign resident status?

    Science.gov (United States)

    2010-04-01

    ... 20 Employees' Benefits 2 2010-04-01 2010-04-01 false When do you lose your foreign resident status... CERTAIN WORLD WAR II VETERANS SVB Qualification and Entitlement Residence Outside the United States § 408.232 When do you lose your foreign resident status? (a) General rule. We consider you to have lost...

  8. 77 FR 55120 - Federal Housing Administration (FHA): Section 232 Healthcare Facility Insurance Program...

    Science.gov (United States)

    2012-09-07

    ... proposed rule at 77 FR 26218, in which it submitted, for public comment, revisions to the Section 232 program regulations. On May 3, 2012, HUD also published a notice at 77 FR 26304, which proposed revisions... the regulatory text but discussed in the preamble to the proposed rule at 77 FR 26222, and...

  9. 48 CFR 52.232-26 - Prompt payment for fixed-price architect-engineer contracts.

    Science.gov (United States)

    2010-10-01

    ... include its TIN on the invoice only if required elsewhere in this contract. (ix) Electronic funds transfer... of Electronic Funds Transfer Information with Offer), contract clause (e.g., 52.232-33, Payment by... interest penalty in accordance with the Office of Management and Budget prompt payment regulations at 5...

  10. 48 CFR 52.232-27 - Prompt payment for construction contracts.

    Science.gov (United States)

    2010-10-01

    ... include its TIN on the invoice only if required elsewhere in this contract. (x) Electronic funds transfer... of Electronic Funds Transfer Information with Offer), contract clause (e.g., 52.232-33, Payment by... interest penalty in accordance with the Office of Management and Budget prompt payment regulations at 5...

  11. 17 CFR 232.105 - Limitation on use of HTML documents and hypertext links.

    Science.gov (United States)

    2010-04-01

    ... 17 Commodity and Securities Exchanges 2 2010-04-01 2010-04-01 false Limitation on use of HTML... Requirements § 232.105 Limitation on use of HTML documents and hypertext links. (a) Electronic filers must... exhibits to Form N-SAR in HTML. (b) Electronic filers may not include in any HTML document hypertext...

  12. CSER 95-003: Exemption from Criticality Alarm System requirement for 232-Z building

    International Nuclear Information System (INIS)

    This CSER establishes an exemption for 232-Z from the requirement for a Criticality Alarm System, because the formation of a critical configuration is not a credible event for any circumstance involving the cleaning out and removal of the Burning Hood and associated equipment

  13. Feeding of the {sup 232}Th levels from the decay of {sup 236}U

    Energy Technology Data Exchange (ETDEWEB)

    Gehrke, R.J. E-mail: rjg@inel.gov; Baker, J.D.; Riddle, C.L

    2002-03-01

    Population of the 6{sup +} 332 keV level in {sup 232}Th from the decay of {sup 236}U was observed for the first time. The 49, 112, and 171 keV {gamma}-ray energies and relative intensities from the decay of {sup 236}U were measured.

  14. 28 CFR 2.32 - Parole to local or immigration detainers.

    Science.gov (United States)

    2010-07-01

    ... 28 Judicial Administration 1 2010-07-01 2010-07-01 false Parole to local or immigration detainers... § 2.32 Parole to local or immigration detainers. (a) When a State or local detainer is outstanding... wishes to parole a prisoner subject to a detainer filed by Federal immigration officials, the...

  15. 49 CFR 232.217 - Train brake tests conducted using yard air.

    Science.gov (United States)

    2010-10-01

    ... 49 Transportation 4 2010-10-01 2010-10-01 false Train brake tests conducted using yard air. 232... Train brake tests conducted using yard air. (a) When a train air brake system is tested from a yard air... reduction of brake pipe air pressure at the same, or slower, rate as an engineer's brake valve. (b) The...

  16. 17 CFR 232.13 - Date of filing; adjustment of filing date.

    Science.gov (United States)

    2010-04-01

    ... REGULATION S-T-GENERAL RULES AND REGULATIONS FOR ELECTRONIC FILINGS General § 232.13 Date of filing... to the applicable technical standards regarding electronic format in the EDGAR Filer Manual; and (iii... otherwise satisfied, all filings submitted by direct transmission commencing on or before 5:30 p.m....

  17. 24 CFR 232.825 - Pro rata refund of insurance premium.

    Science.gov (United States)

    2010-04-01

    ... 24 Housing and Urban Development 2 2010-04-01 2010-04-01 false Pro rata refund of insurance... ASSISTED LIVING FACILITIES Contract Rights and Obligations Premiums § 232.825 Pro rata refund of insurance... rata portion of the current annual loan insurance premium theretofore paid which is applicable to...

  18. 230,232Th in milk, meat, and grain in Korea

    International Nuclear Information System (INIS)

    The concentrations of natural radioisotopes 230Th and 232Th in Korean foods were measured by the method of calcium oxalate co-precipitation in addition to the conventional anion-exchange method and alpha spectroscopic measurement. The 230Th concentrations (mBq/kg-fresh) in Korean foods were found to be as follows: milk 0.14-2.45, pork 2.98-8.97, beef 1.94-9.80, chicken 1.22-13.0, rice 0.43-2.35, wheat 0.53-14.4, and soybeans, 8.44-91.6. The 232Th concentrations (mBq/kg-fresh) in Korean foods were found to be as follows: milk 0.01-2.46, pork 0.28-9.32, beef 1.02-5.34, chicken 0.56-4.98, rice 0.32-2.54, wheat 0.53-20.0, and soybeans, 2.30-42.2. The annual internal dose of Th was also estimated. The annual internal dose of 230Th and 232Th in milk was about 0.006 μSv/yr and much lower than that of other countries because of the low intake of milk in Korea compared to other countries. The annual internal dose of 230Th and 232Th in the rice was about 0.043 μSv/yr and highest because rice is the staple food of Koreans. (author)

  19. 48 CFR 252.232-7003 - Electronic submission of payment requests and receiving reports.

    Science.gov (United States)

    2010-10-01

    ... PROVISIONS AND CONTRACT CLAUSES Text of Provisions And Clauses 252.232-7003 Electronic submission of payment... administering the contract for payment has determined, in writing, that electronic submission would be unduly... non-electronic payment requests using the method or methods specified in Section G of the contract....

  20. 17 CFR 232.311 - Documents submitted in paper under cover of Form SE.

    Science.gov (United States)

    2010-04-01

    ... section, may be filed up to six business days prior to, or on the date of filing of, the electronic format... EXCHANGE COMMISSION REGULATION S-T-GENERAL RULES AND REGULATIONS FOR ELECTRONIC FILINGS Preparation of Electronic Submissions § 232.311 Documents submitted in paper under cover of Form SE. Form SE (§§ 239.64,...

  1. 232Th and 238U neutron emission cross section calculations and analysis of experimental data

    International Nuclear Information System (INIS)

    In this study, pre-equilibrium neutron-emission spectra produced by (n,xn) reactions on nuclei 232Th and 238U have been calculated. Angle-integrated cross sections in neutron induced reactions on targets 232Th and 238U have been calculated at the bombarding energies up to 18 MeV. We have investigated multiple pre-equilibrium matrix element constant from internal transition for 232Th (n,xn) neutron emission spectra. In the calculations, the geometry dependent hybrid model and the cascade exciton model including the effects of pre-equilibrium have been used. In addition, we have described how multiple pre-equilibrium emissions can be included in the Feshbach-Kerman-Koonin (FKK) fully quantum-mechanical theory. By analyzing (n,xn) reaction on 232Th and 238U, with the incident energy from 2 Me V to 18 Me V, the importance of multiple pre-equilibrium emission can be seen cleady. All calculated results have been compared with experimental data. The obtained results have been discussed and compared with the available experimental data and found agreement with each other

  2. 49 CFR 232.107 - Air source requirements and cold weather operations.

    Science.gov (United States)

    2010-10-01

    ... 49 Transportation 4 2010-10-01 2010-10-01 false Air source requirements and cold weather... AND OTHER NON-PASSENGER TRAINS AND EQUIPMENT; END-OF-TRAIN DEVICES General Requirements § 232.107 Air source requirements and cold weather operations. (a) Monitoring plans for yard air sources. (1)...

  3. FUSION-LIKE PROCESSES IN THE N-14+TH-232 REACTION AT 30 MEV NUCLEON

    NARCIS (Netherlands)

    LEEGTE, HKW; BOONSTRA, AL; HINNEFELD, JD; KOLDENHOF, EE; SIEMSSEN, RH; SIWEKWILCZYNSKA, K; SOSIN, Z; WILCZYNSKI, J; WILSCHUT, HW

    1992-01-01

    Fusionlike processes were studied in the N-14 + Th-232 reaction at 30 MeV per nucleon. Partition of the fusionlike cross section was determined by detecting nonequilibrium charged particles with an array of phoswich detectors (plastic wall) in coincidence with fission fragments for which the folding

  4. Architectural, Mechanical, Electrical, Plumbing, and Site Documents Associated with Sustainability Base, N232

    Science.gov (United States)

    Grymes, Rosalind A.; Martin, Rodney Alexander; Dianati, Soheila

    2016-01-01

    These files contain more precise and accurate representations of the architectural, mechanical, electrical, plumbing, and site information pertaining to Sustainability Base, aka Collaborative Support Facility, aka N232. These supersede the 'bid' drawings released in STI 8112 previously. They are useful for NASA researchers and collaborators in modeling the performance characteristics of the facility. Otherwise, they do not contain new data.

  5. 29 CFR 779.232 - Franchise or other arrangements which create a larger enterprise.

    Science.gov (United States)

    2010-07-01

    ... Apply; Enterprise Coverage Leased Departments, Franchise and Other Business Arrangements § 779.232... business in the one granting the franchise, the result is to place the dealer in a larger enterprise with... franchisor desired to extend its business through the operation of associated franchise stores,...

  6. Optical isolation and surge protection of RS-232 port%RS-232端口光电隔离型电涌保护器

    Institute of Scientific and Technical Information of China (English)

    王金虎; 李祥超; 刘晓东; 黄鹏良

    2011-01-01

    根据气体放电管和瞬态抑制二极管的保护特性,合理选择退耦元件参数,实现多级SPD间的能量配合,并结合光纤的保护性能设计RS-232接口的保护电路.最后利用雷电冲击试验平台LST-6kV/3 kA、ICGS冲击平台以及DF1641C函数发生器对保护电路进行实验,以验证设计的方案.实验结果表明:在加上保护器件后,通信端口的抗雷电过压能力得到了很大的提高,并且加入该保护电路以后基本不会对原电路产生插入损耗.%Lightning over-voltages are the important reasons for losses in communication port, which make it neces-sary and urgent to study into the lightning protection of communication port. According to the protection characteris-tics of gas discharge tube and transient voltage suppressor, the decoupling components are selected carefully to a-chieve the rational energy correspondence between multi-level SPD. Besides that,optical design is also considered to design protective circuit of RS-232 port. Finally,in order to verify the design scheme,the lightning impact platform called LST-6 kV/3 kA and ICGS and function generator called DF1641C are employed for the experiments. The ex-periments show that bearing capacity of lightning over-voltage of communication port RS-232 has been greatly im-proved and will not produce insertion loss to original circuit by adding the protection circuit.

  7. Measurement of 232Th(, ) and 232Th(, 2) cross-sections at neutron energies of 13.5, 15.5 and 17.28 MeV using neutron activation techniques

    Indian Academy of Sciences (India)

    Sadhana Mukerji; H Naik; S V Suryanarayana; S Chachara; B S Shivashankar; V Mulik; Rita Crasta; Sudipta Samanta; B K Nayak; A Saxena; S C Sharma; P V Bhagwat; K K Rasheed; R N Jindal; S Ganesan; A K Mohanty; A Goswami; P D Krishnani

    2012-08-01

    The 232Th(, ) reaction cross-section at average neutron energies of 13.5, 15.5 and 17.28 MeV from the 7Li(, ) reaction has been determined for the first time using activation and off-line -ray spectrometric technique. The 232Th(, 2) cross-section at 17.28 MeV neutron energy has also been determined using the same technique. The experimentally determined 232Th(, ) and 232Th(, 2) reaction cross-sections from the present work were compared with the evaluated data of ENDF/BVII and JENDL-4.0 and were found to be in good agreement. The present data, along with literature data in a wide range of neutron energies, were interpreted in terms of competition between 232Th(, ), (, ), (, ) and (, ) reaction channels. The 232Th(, ) and 232Th(, 2) reaction cross-sections were also calculated theoretically using the TALYS 1.2 computer code and were found to be in good agreement with the experimental data from the present work but were slightly higher than the literature data at lower neutron energies.

  8. Measurement of the generation ratio of 233U and the average radiation capture cross section of 232Th with 232ThO2 irradiated by fast neutrons

    International Nuclear Information System (INIS)

    Background: Thorium-Uranium cycle plays an important role in the future's power production technology. Nuclear data involved are urgently needed for engineering design and other purposes since there are obvious differences between the existing evaluated data. Macroscopic neutron integral experiment can be used as a good tool to survey the confusion. Purpose: Macroscopic neutron integral experiment based on radioactive method was carried out to measure the generation ratio of 233U nuclide and the average radiation capture cross section of 232Th while a ThO2 sample was irradiated by fast neutrons leakage from a fast critical facility. We expect that these data can be used as a reference for the research of Th-U cycle. Methods: Radiation capture reactions of 232Th nuclides occur when the nuclides are irradiated by neutrons. 233U nuclides will be generated after two cascade decays by emitting beta rays from the activation products, which are 233Th nuclides. The ThO2 sample was prepared as a slice of 20 mm×10 mm from 0.743 36-g ThO2 powders of 99.9% enriched. The neutron flux was measured by activation method which was 4.07x109 cm-2·s-1 at the sample's irradiation position while the facility worked at the power level of 180 watts. The leakage neutrons' energy distribution was calculated by MC method and it is very close to the fission spectrum with the averaged energy of 1.42 MeV. After irradiation and then a period of cooling time the gamma rays emitted from the sample were measured by an HPGe spectrometer which had been pre-calibrated. From these data the activity of 233Pa was calculated and then the generation ratio of 233U and the average radiation capture cross section of 232Th were calculated. The measured average radiation capture cross section was compared with the cross sections calculated based on the ENDFB-VH.1, CENDL-3.1, JENDL-4.0, BROND2.2 databases. Results: The measured generation ratio of 233U was 4.01×10-12 with an uncertainty of 6

  9. Determination of 232Th, 230Th and 228Th in liquid effluents from uranium mining

    International Nuclear Information System (INIS)

    A liquid scintillator αlpha spectrometer was built for the determination of Th-228, Th-230 and Th-232 in liquid effluents from Uranium mines and mills. The resolution of the αlpha spectrometer was found to be 200-300 KeV, when the scintillator was 8% T0P0, 0,77% scintimix-4 (91% PP0 and 9% Dimetil-P0P0P) and 10% of naphthalene in toluene. Aliquat-336 in xylene (30% v/v) was used to separate the thorium isotopes from other interfering radionuclides (U-238, U-234, Ra-226, Po-210). Under the extraction experimental conditions, the detection limits were 1,2 pCi/1 for Th-232, 1,2 pCi/1 for Th-230 and 0,9 pCi/1 for Th-228, for 1000 minutes of counting time. (author)

  10. 226Ra, 232Th and 40K analysis in water samples from Assiut, Egypt

    International Nuclear Information System (INIS)

    The activity concentrations of 226Ra, 232Th and 40K were determined in water samples, using 2”x 2” NaI(Tl) scintillation detector. Water activity ranges from 0.07 to 0.59 Bq L−1 for 226Ra, 0.05 to 0.37 Bq L−1 for 232Th and 3.25 to 8.72 Bq L−1 for 40K with mean values of 2.64, 2.22 and 119.50 Bq L−1, respectively. As far as the measured gamma radionuclides is concerned, the mean annual effective doses for all analyzed samples of water are in the range of 0.02–0.08, 0.03-0.17 and 0.03-0.10 mSv yr-1 for infants, children and adults, respectively, all being lower than the reference level of the committed effective dose recommended by the WHO.

  11. Absence of {sup 232,230,228}Th enhancement decay by ultrasound exposure

    Energy Technology Data Exchange (ETDEWEB)

    Aupiais, J. [CEA DAM DIF, Arpajon (France); Cousin, V.; Nikitenko, S.I.; Pflieger, R. [Marcoule Institute for Separation Chemistry, ICSM, UMR 5257, Bagnols-sur-Ceze (France); Moisy, P. [CEA, Bagnols-sur-Ceze (France). RadioChemistry and Processes Dept.

    2013-08-01

    We report on our attempt to reproduce the {sup 228}Th decay enhancement under the effect of power ultrasound claimed recently in the literature. The evolution of natural thorium isotopic composition ({sup 232}Th, {sup 230}Th, and {sup 228}Th) in various aqueous solutions submitted to 20 kHz power ultrasound (0.18 W mL{sup -1}, 20 C, Ar). The radioactivities of the three isotopes of thorium ({sup 232}Th, {sup 230}Th and {sup 228}Th) were followed by a liquid scintillation counting technique. No change was detected during ultrasonic irradiation. Our results demonstrate that under the studied conditions the rate of Th isotopes radioactive decay is not modified under the effect of ultrasound on aqueous solutions of thorium salts. (orig.)

  12. Fractional absorption in gastrointestinal tract of 232Th by ingestion for Chinese man

    International Nuclear Information System (INIS)

    Objective: To estimate fractional absorption in gastrointestinal tract (f1) of 232Th by ingestion for the Chinese male adults. Methods: According to f1 calculation method in literature and results of Th concentrations in dietary foods and organ or tissues for the Chinese male adults, obtained in recent years, f1 values were estimated from the median and mean Th concentrations and compared each other. Results: the f1 value from the median and mean Th concentrations was 0.00048 and 0.00028 respectively. Conclusion: The f1 of 232Th by ingestion for the Chinese male adults should be adopted as 0.00048, being lower than estimated result from the world reference concentrations in UNSCEAR 2000 Report, but quite near to the relevant reported value from Asian countries, such as India or Japan, and supporting the latest recommended value 0.0005 by ICRP too

  13. Standard guide for the determination of uranium-232 in uranium hexafluoride

    CERN Document Server

    American Society for Testing and Materials. Philadelphia

    2006-01-01

    1.1 This method covers the determination of 232U in uranium hexafluoride by alpha spectrometry. 1.2 This standard does not purport to address all of the safety concerns, if any, associated with its use. It is the responsibility of the user of this standard to establish appropriate safety and health practices and to determine the applicability of regulatory limitations prior to use.

  14. Fission Product Decay Heat Calculations for Neutron Fission of 232Th

    Science.gov (United States)

    Son, P. N.; Hai, N. X.

    2016-06-01

    Precise information on the decay heat from fission products following times after a fission reaction is necessary for safety designs and operations of nuclear-power reactors, fuel storage, transport flasks, and for spent fuel management and processing. In this study, the timing distributions of fission products' concentrations and their integrated decay heat as function of time following a fast neutron fission reaction of 232Th were exactly calculated by the numerical method with using the DHP code.

  15. The Design Points of RS232 -RS422/RS485/TLL Signal Converter%RS232-RS422/RS485/TLL信号转换器设计

    Institute of Scientific and Technical Information of China (English)

    苏燕; 周士龙

    2012-01-01

    主要介绍了RS232-RS422/485信号转换器在窃电电路、自动方向转换电路、RS232信号补偿电路的设计要点,提出了将RS422接口与TLL接口兼容使用的方法。%This article mainly introduces design points of the RS232 -RS422/485 signal converter's getting power supply from signal pins circuit, automatic direction of transform circuit and RS232 signal compensation circuit. It puts forward the RS422 interface and TLL interface compatibility methods

  16. Decontamination and decommissioning assessment for the Waste Incineration Facility (Building 232-Z) Hanford Site, [Hanford], WA

    International Nuclear Information System (INIS)

    Building 232-Z is an element of the Plutonium Finishing Plant (PFP) located in the 200 West Area of the Hanford Site. From 1961 until 1972, plutonium-bearing combustible materials were incinerated in the building. Between 1972 and 1983, following shutdown of the incinerator, the facility was used for waste segregation activities. The facility was placed in retired inactive status in 1984 and classified as a Limited Control Facility pursuant to DOE Order 5480.5, Safety of Nuclear Facilities, and 6430.1A, General Design Criteria. The current plutonium inventory within the building is estimated to be approximately 848 grams, the majority of which is retained within the process hood ventilation system. As a contaminated retired facility, Building 232-Z is included in the DOE Surplus Facility Management Program. The objective of this Decontamination and Decommissioning (D ampersand D) assessment is to remove Building 232-Z, thereby elmininating the radiological and environmental hazards associated with the plutonium inventory within the structure. The steps to accomplish the plan objectives are: (1) identifying the locations of the most significant amounts of plutonium, (2) removing residual plutonium, (3) removing and decontaminating remaining building equipment, (4) dismantling the remaining structure, and (5) closing out the project

  17. Distribution of 137Cs, 40K, 238U and 232Th in soils from Northern Venezuela

    International Nuclear Information System (INIS)

    More than one hundred undisturbed soil samples form Northern Venezuela and the islands of Margarita and Los Roques have been analyzed for 137Cs, 40K, 238U and 232Th by γ-ray spectroscopy. The specimens were taken from between 5-10 cm below the earth's surface. Thus, they are valid not only for the 137Cs deposition studies but also for the estimation of the natural γ-ray dose from primordial radionuclides that form the terrestrial component. The concentrations of 40K was directly determined from its 1461 keV γ-ray, while those of 137Cs, 238U and 232Th were performed using a γ-ray from one of their daughter radionuclides: the 661 keV γ-ray of 137mBa for 137Cs, the 1760 keV γ-ray of 214Bi for 238U and the 2620 keV γ-ray of 208Tl for 232Th. Finally, the concentration values were compared with those of global estimates. (author) 15 refs.; 4 figs.; 2 tabs

  18. Radiationless transition probabilities in muonic 208Pb, 232Th, and 238U

    International Nuclear Information System (INIS)

    The probabilities for non-radiative (n.r.) excitations Pn.r. in the muonic nuclides 208Pb, 232Th, and 238U have been determined for (μ-, γγ)-measurements by comparing the intensities of muonic X-ray transitions in single and coincidence spectra. The value of Pn.r. (3p→1s), measured for the first time, is about 90% for the actinides 232Th and 238U, but only about 8% for 208Pb. The value of Pn.r. (3d→1s) is found to be 10% for 233Th, 13% for 238U, and about 4% for 208Pb. For 208Pb a vanishing strength of the n.r. decay of the 2p-level is found, while for 232Th and for 238U n.r. strengths of about 20% and 26%, respectively, are observed. By regarding two subcomplexes of the 2p→1s transitions leading to different mean excitation energies the n.r. transition probabilities were found to be different for 238U only, 21.6% and 31.1%, respectively. (orig.)

  19. Inhaled americium dioxide

    International Nuclear Information System (INIS)

    This project includes experiments to determine the effects of Zn-DTPA therapy on the retention, translocation and biological effects of inhaled 241AmO2. Beagle dogs that received inhalation exposure to 241AmO2 developed leukopenia, clincial chemistry changes associated with hepatocellular damage, and were euthanized due to respiratory insufficiency caused by radiation pneumonitis 120 to 131 days after pulmonary deposition of 22 to 65 μCi 241Am. Another group of dogs that received inhalation exposure to 241AmO2 and were treated daily with Zn-DTPA had initial pulmonary deposition of 19 to 26 μCi 241Am. These dogs did not develop respiratory insufficiency, and hematologic and clinical chemistry changes were less severe than in the non-DTPA-treated dogs

  20. 17 CFR 232.312 - Accommodation for certain information in filings with respect to asset-backed securities.

    Science.gov (United States)

    2010-04-01

    ... ELECTRONIC FILINGS Preparation of Electronic Submissions § 232.312 Accommodation for certain information in...)(3) and (a)(4) of this section, the five-year period shall commence from the filing date of...

  1. Neutron inelastic-scattering cross sections of 232Th, 233U, 235U, 238U, 239Pu and 240Pu

    International Nuclear Information System (INIS)

    Differential-neutron-emission cross sections of 232Th, 233U, 235U, 238U, 239Pu and 240Pu are measured between approx. = 1.0 and 3.5 MeV with the angle and magnitude detail needed to provide angle-integrated emission cross sections to approx. 232Th, 233U, 235U and 238U inelastic-scattering values, poor agreement is observed for 240Pu, and a serious discrepancy exists in the case of 239Pu

  2. S232祖克浆纱机的改造实践%Reformation Practice of SUCKER S232 Sizing Machine

    Institute of Scientific and Technical Information of China (English)

    刘安君; 窦海萍

    2009-01-01

    为解决祖克S232浆纱机织轴卷绕故障率高、烘燥温度不稳定、压浆力调节装置失控、经轴退绕张力不稳定等问题,进行了技术改造。通过采用多单元技术对织轴卷绕装置进行了两单元改造,对温控系统、压浆力调节装置以及经轴退绕装置采用了可编程PLC控制技术,改造后提高了机器的自动化程度,降低了设备故障率,提高了浆纱质量。

  3. Studies on {sup 232}Th and {sup 238}U levels in marine algae collected from the coast of Niigata Prefecture

    Energy Technology Data Exchange (ETDEWEB)

    Kato, Kenji; Tonouchi, Shigemasa; Maruta, Fumiyuki; Ebata, Hidekazu [Niigata Prefectural Inst. of Public Health and Environmental Sciences (Japan)

    2001-12-01

    To evaluate the properties of algae to concentrate radioactive elements, 14 species of algae like Sargassum were collected in the Prefecture and analyzed for their {sup 232}Th and {sup 238}U levels with Yokogawa HP4500 ICP-MS apparatus. The places of collection included those near the water discharge of an atomic power station. Mean {sup 232}Th and {sup 238}U levels were found to be 120 and 260 ng/g dry wt, respectively, and Phaeophyta showed more than several times higher {sup 238}U level than Chlorophyta and Rhodophyta. There was no clear difference in {sup 232}Th levels. No difference between places of collection was observed in Sargassum {sup 232}Th or {sup 238}U level. Adsorption of {sup 232}Th particle to and incorporation of soluble {sup 238}U into algae body were suggested. Mean {sup 232}Th and {sup 238}U radioactivities were found 73 and 510 {mu}Bq/g wet wt, respectively, and the respective annual committed effective doses, 0.2 and 0.3 {mu}Sv, calculated from those values were confirmed to be enough lower than the annual public dose limit, 1 mSv. (K.H.)

  4. Recovery of Americium-241 from lightning rod by the method of chemical treatment; Recuperacion del Americio-241 provenientes de los pararrayos por el metodo de tratamiento quimico

    Energy Technology Data Exchange (ETDEWEB)

    Cruz, W.H., E-mail: wcruz@ipen.gob.pe [Instituto Peruano de Energia Nuclear (GRRA/IPEN), Lima (Peru). Division de Gestion de Residuos Radiactivos

    2013-07-01

    About 95% of the lightning rods installed in the Peruvian territory have set in their structures, pose small amounts of radioactive sources such as Americium-241 ({sup 241}Am), fewer and Radium 226 ({sup 226}Ra) these are alpha emitters and have a half life of 432 years and 1600 years respectively. In this paper describes the recovery of radioactive sources of {sup 241}Am radioactive lightning rods using the conventional chemical treatment method using agents and acids to break down the slides. The {sup 241}Am recovered was as excitation source and alpha particle generator for analysing samples by X Ray Fluorescence, for fixing the stainless steel {sup 241}Am technique was used electrodeposition. (author)

  5. Partitioning studies in China and the separation of americium and fission product rare earths with dialkyl phosphinic acid and its thio-substituted derivatives

    International Nuclear Information System (INIS)

    Studies on the TRPO extractions process for recovering actinides from highly active waste (HAW) and its application to the pretreatment of Chinese HAW are described. The removal of Sr by di-cyclohexyl 18 crown 6 and the removal of Cs by spherical titanium ferrous hexa-cyanate from acidic waste are also described. Results of the extraction of trivalent americium and fission product rare earths (FPREs) by dialkyl-phosphinic, dialkyl-mono-thio-phosphinic and dialkyl-di-thio-phosphinic acids are reported. Dialkyl-thio-phosphinic acid (commercial product Cyanex 301, alkyl =2, 4, 4-methyl-pentyl) shows very high selectivity towards Am. Using 1M Cyanex 301 -kerosene as extractant, 99.9 % Am can be separated from 0.5M(Pr+Nd)(NO3)3 solution with 3-4 extraction stages and 3-4 scrubbing stages. (authors)

  6. Theoretical and experimental study of the bio-geochemical behaviour of americium 241 in simplified rhizosphere conditions. Application to a calcareous agricultural soil

    International Nuclear Information System (INIS)

    Americium 241, is one of the most radio-toxic contaminant produced during the nuclear fuel cycle. It can be found in all environmental compartments, in particular the soils. The main goals of this study are to identify, quantify and model the effect of the main factors controlling the mobility of 241Am in the rhizosphere and the agricultural soils. The physico-chemical parameters of the soil and of the soil solution, the potential role of microorganisms on the sorption-desorption processes, and the speciation of americium in solution have been more particularly studied. 241Am remobilization has been studied at the laboratory using leaching experiments performed in controlled conditions on reworked calcareous soils artificially contaminated with 241Am. The soil samples have been washed out in different hydrodynamic conditions by solutions with various compositions. The eluted solution has been analyzed (pH, conductivity, ionic composition, Fetot, organic acids, 241Am) and its bacterial biomass content too. The overall results indicate that 241Am remobilization is contrasted and strongly linked with the condition under study (pH, ionic strength, glucose and/or citrate concentration). Therefore, a solution in equilibrium with the soil or containing small exudate concentrations (10-4 M) re-mobilizes only a very small part of the americium fixed on the solid phase. The desorption of 241Am corresponds to a solid/liquid coefficient of partition (Kd) of about 105 L.kg-1. A significant addition of glucose induces an important dissolution of soil carbonates by the indirect action of microorganisms, but does not significantly favor the 241Am remobilization. On the other hand, the presence of strong citrate concentrations (≥ 10-2 M) allows 300 to 10000 time greater re-mobilizations by the complexing of 241Am released after the dissolution of the carrying phases. Finally, the colloidal transport of 241Am has been systematically observed in a limited but significant extend and

  7. 基于RS232-USB转换器及LabVIEW平台下温湿度采集系统的设计%Design of test program for RS232-USB converter

    Institute of Scientific and Technical Information of China (English)

    周静; 张蕾; 南洋

    2012-01-01

    本文将RS232-USB转换器及虚拟仪器技术应用于温湿度测量中,以LabVIEW为软件开发平台,以计算机为核心,配上传感器、RS232-LJSB转换器和相应软件,针对室内环境的温湿度进行实时精确的采集及测量,编写了数据处理程序和人机交互界面,将结果通过人机交互界面以数字的方式进行实时显示,显示了虚拟仪器技术在温湿度测量中应用的灵活性和其功能的强大性,同时体现了RS232-USB转换器的RS232串行口至USB口转换功能的稳定性。实验表明,该系统能实时准确地采集温湿度信息,并通过RS232口-USB口显示至PC上,达到了可视化的效果。%The application of the RS232-USB converter and virtual instrument in the measurement of temperature and humidity in the article, with LabVIEW as software development platform, using the computer as the core, with the sensor, the RS232-USB converter and the corresponding software, the indoor temperature and humidity of the environment, precise real-time collection and measurement, a data processing program and human-computer interaction interface, will the results man-machine interface to the digital approach for real-time display, display of virtual instrument technology in the measurement of temperature and humidity application flexibility and its function of the powerful ,At the same time reflects the RS232-USB converter RS232 serial port to the USB conversion function stability .Based on the experiment, the system can real-time and accurate acquisition of temperature and humidity information, and through RS232 - USB port display to the PC, achieved the visual effect.

  8. Safe handling of kilogram amounts of fuel-grade plutonium and of gram amounts of plutonium-238, americium-241 and curium-244

    International Nuclear Information System (INIS)

    During the past 10 years about 600 glove-boxes have been installed at the Institute for Transuranium Elements at Karlsruhe. About 80% of these glove-boxes have been designed and equipped for handling 100-g to 1-kg amounts of 239Pu containing 8-12% 240Pu (low-exposure plutonium). A small proportion of the glove-boxes is equipped with additional shielding in the form of lead sheet or lead glass for work with recycled plutonium. In these glove-boxes gram-amounts of 241Am have also been handled for preparation of Al-Am targets using tongs and additional shielding inside the glove-boxes themselves. Water- and lead-shielded glove-boxes equipped with telemanipulators have been installed for routine work with gram-amounts of 241Am, 243Am and 244Cm. A prediction of the expected radiation dose for the personnel is difficult and only valid for a preparation procedure with well-defined preparation steps, owing to the fact that gamma dose-rates depend strongly upon proximity and source seize. Gamma radiation dose measurements during non-routine work for 241Am target preparation showed that handling of gram amounts leads to a rather high irradiation dose for the personnel, despite lead or steel glove-box shielding and shielding within the glove-boxes. A direct glove-hand to americium contact must be avoided. For all glove-handling of materials with gamma radiation an irradiation control of the forearms of the personnel by, for example, thermoluminescence dosimeters is necessary. Routine handling of americium and curium should be executed with master-slave equipment behind neutron and gamma shielding. (author)

  9. Monitoring of 232Th in soil of the state of Pernambuco, Brazil

    Energy Technology Data Exchange (ETDEWEB)

    Santos Junior, Jose Araujo dos; Silva, Cleomacio Miguel da; Silveira, Sueldo Vita; Amaral, Romilton dos Santos [Pernambuco Univ., Recife, PE (Brazil). Dept. de Energia Nuclear. Grupo de Estudos em Radioprotecao e Radioecologia (GERAR)]. E-mail: jaraujo@ufpe.br; Cardoso, Jorge Joao Ricardo Ferreira [Pernambuco Univ., Recife, PE (Brazil). Dept. de Geologia]. E-mail: jcardoso@ufpe.br

    2005-07-01

    where the control of radionuclides in the environment is of extreme importance for attaining information on potential sources of radioactive contamination. The gamma spectrometry with high resolution detector is a rapid and efficient method in the determination of natural radionuclides in environment samples. Using the gamma spectrometry with HPGe, it was possible to measure the radiological concentrations of {sup 232}Th in seventy eight soil samples, collected in an area of approximately 40,000 m{sup 2}, around a natural radioactive occurrence, located in the rural region of the state Pernambuco, Brazil. The samples of 200 g, were reduced to a granulometry less than 63 {mu}m, homogenized, conditioned in hermetically sealed polyethylene containers for thirty days, and measured in the laboratory for 43,200 seconds, each. The measurements of the activities of {sup 232}Th were based on the gamma emissions of the photo peaks at 338 keV and 911 keV of {sup 228}Ac in secular radioactive balance, and allowed the evaluation of the distribution of these radionuclides in the environment. For the calculation of the specific activities of {sup 232}Th, the average of the rates of counting in the energies of 338 keV and 911 keV was used (discrepancy of approximately 5 %). The values of the measured activities have variations of 77 to 423 Bq.kg{sup -1} (arithmetic mean 227 Bq.kg{sup -1}; median 217 Bq.kg{sup -1}). The average factor concentration was approximately 6. (author)

  10. Hard synchrotron BL Lacs: the case of 1ES 1101-232

    OpenAIRE

    Wolter, Anna; Ghisellini, Gabriele; Tagliaferri, Gianpiero; Tavecchio, Fabrizio; Caccianiga, Alessandro

    2000-01-01

    The bright X-ray selected BL Lac object 1ES1101--232 shows a flat X-ray spectrum, making it detectable with high statistics over the wide BeppoSAX energy range. We have observed it in two different epochs with BeppoSAX, and found a variation of the flux of about 30% that can be explained by a change in the spectral index above the synchrotron peak. We present here the data and infer limits on the strength of the magnetic field based on models of emission for High-frequency peaked BL Lacs.

  11. Spatial variability of initial 230Th/ 232Th in modern Porites from the inshore region of the Great Barrier Reef

    Science.gov (United States)

    Clark, Tara R.; Zhao, Jian-xin; Feng, Yue-xing; Done, Terry J.; Jupiter, Stacy; Lough, Janice; Pandolfi, John M.

    2012-02-01

    The main limiting factor in obtaining precise and accurate uranium-series (U-series) ages of corals that lived during the last few hundred years is the ability to constrain and correct for initial thorium-230 ( 230Th 0), which is proportionally much higher in younger samples. This is becoming particularly important in palaeoecological research where accurate chronologies, based on the 230Th chronometer, are required to pinpoint changes in coral community structure and the timing of mortality events in recent time (e.g. since European settlement of northern Australia in the 1850s). In this study, thermal ionisation mass spectrometry (TIMS) U-series dating of 43 samples of known ages collected from living Porites spp. from the far northern, central and southern inshore regions of the Great Barrier Reef (GBR) was performed to spatially constrain initial 230Th/ 232Th ( 230Th/ 232Th 0) variability. In these living Porites corals, the majority of 230Th/ 232Th 0 values fell within error of the conservative bulk Earth 230Th/ 232Th atomic value of 4.3 ± 4.3 × 10 -6 (2 σ) generally assumed for 230Th 0 corrections where the primary source is terrestrially derived. However, the results of this study demonstrate that the accuracy of 230Th ages can be further improved by using locally determined 230Th/ 232Th 0 values for correction, supporting the conclusion made by Shen et al. (2008) for the Western Pacific. Despite samples being taken from regions adjacent to contrasting levels of land modification, no significant differences were found in 230Th/ 232Th 0 between regions exposed to varying levels of sediment during river runoff events. Overall, 39 of the total 43 230Th/ 232Th 0 atomic values measured in samples from inshore reefs across the entire region show a normal distribution ranging from 3.5 ± 1.1 to 8.1 ± 1.1 × 10 -6, with a weighted mean of 5.76 ± 0.34 × 10 -6 (2 σ, MSWD = 8.1). Considering the scatter of the data, the weighted mean value with a more

  12. Implications of a DK Molecule at 2.32 GeV

    CERN Document Server

    Barnes, T; Lipkin, H J

    2003-01-01

    We discuss the implications of a possible quasinuclear DK bound state at 2.32 GeV. Evidence for such a state was recently reported in D_s^+pi^o by the BaBar Collaboration. We first note that a conventional quark model c-sbar assignment is implausible, and then consider other options involving multiquark systems. An I=0 c sbar n nbar baryonium assignment is one possibility. We instead favor a DK meson molecule assignment, which can account for the mass and quantum numbers of this state. The higher-mass scalar c-sbar state expected at 2.48 GeV is predicted to have a very large DK coupling, which would encourage formation of an I=0 DK molecule. Isospin mixing is expected in hadron molecules, and a dominantly I=0 DK state with some I=1 admixture could explain both the narrow total width of the 2.32 GeV state as well as the observed decay to D_s^+ pi^o. Additional measurements that can be used to test this and related scenarios are discussed.

  13. Studies of positron electron pair production in {sup 238}U + {sup 232}Th

    Energy Technology Data Exchange (ETDEWEB)

    Ahmad, I.; Back, B.B.; Betts, R.R. [and others

    1995-08-01

    Following the non-observation of sharp sum-energy lines in our earlier {sup 238}U + {sup 181}Ta measurements, it was decided to pursue measurements of the {sup 238}U + {sup 232}Th system which, in the previously published work, showed the most striking evidence for near-equal-energy back-to-back pairs leading to sharp sum-energy lines. Following the refurbishing of the APEX silicon arrays and extensive tests of the rotating target wheel assembly, a major positron run took place in November 1994. Rolled 1-mg/cm{sub 2} {sup 232}Th targets were bombarded with 5.95-MeV/u {sup 238}U. The target rotation allowed up to 2 pnA of beam to be used without serious deterioration of the targets. Over 300,000 pairs were accumulated, representing an order-of-magnitude improvement in statistics over the previously published results. Preliminary analysis shows no evidence for the sharp lines at a cross section level orders of magnitude below those previously reported. The analysis of these data is currently being completed in preparation for publication.

  14. High resolution photofission measurements in 238U and 232Th. Final report

    International Nuclear Information System (INIS)

    A novel technique for measuring the photofission cross section with very high photon energy resolution has been developed. The photons are obtained from selected resonances in the (p,γ) reaction on various light nuclei. The photon energy resolution approaches 200 eV in favorable cases. The photon energy spread at each (p,γ) resonance is approx.20 keV on the average. Measurements of the photo-fission cross sections of 232Th and 238U have been carried out in the energy range from 5.8 to 12 MeV. Intermediate structure has been found in both nuclei at excitation energies around 6 MeV. Various properties of this structure, such as average areas of resonances, their spacing, width, and the underlying bakground, as well as the experimental fission probability averaged over the intermediate structure have been found to agree with theoretical predictions based on a double-humped fission barrier. In the case of 232Th, the feature of this barrier, a rather high first hump and a deep secondary well, are quite different from those predicted by current theoretial barrier calculations. 13 refs., 4 figs., 3 tabs

  15. Natural activities of {sup 238}U, {sup 232}Th and {sup 40}K in building materials

    Energy Technology Data Exchange (ETDEWEB)

    Ibrahim, N. [Department of Physics, University of Malaya, 50603 Kuala Lumpur (Malaysia)

    1999-05-01

    Seven kinds of building materials were analysed for {sup 238}U, {sup 232}Th and {sup 40}K using a direct {gamma}-counting method. The activity concentrations measured for {sup 238}U (30-448 Bq kg{sup -1}) and {sup 40}K (328-7541 Bq kg{sup -1}) were greater than the world average activity for soil (25 and 370 Bq kg{sup -1}, respectively) for all building materials analysed, while the activity concentrations of {sup 232}Th were found to exceed the average of 25 Bq kg{sup -1} (soil) for red-clay brick (51 Bq kg{sup -1}) and ceiling asbestos sheet materials (162 Bq kg{sup -1}). The calculated Ra equivalent activities (Ra{sub eq}) for all materials are higher than the world average value for soil (89 Bq kg{sup -1}). For red-clay brick and ceiling asbestos, the Ra{sub eq} values are found to exceed the limit of 370 Bq kg{sup -1}, equivalent to a {gamma}-dose of 1.5 mSv yr{sup -1}. (Copyright (c) 1999 Elsevier Science B.V., Amsterdam. All rights reserved.)

  16. Laboratory Bioaccumulation, Depuration And Total Dose Rate Of Waterborne Th-232 In Freshwater Fish Of Anabas Testudineus

    International Nuclear Information System (INIS)

    Preliminary results on the study of bioaccumulation, depuration and total dose rate of Th-232 in the whole body of Anabas testudineus are presented. The objective of this study was to evaluate the effect of Th-232 concentration activity on the laboratory bioaccumulation, depuration and total dose rate in Anabas testudineus. Anabas testudineus adults were exposed to different waterborne Th-232 levels: 0 BqL-1 (control), 50 BqL-1 and 100 BqL-1 for 30 day (uptake phase), followed by exposure to radionuclide-free water for 30 days (loss phase). Radionuclide concentration ratios between the whole body levels and water levels, percentage of Th-232 remaining in fish were calculated and total dose rates using ERICA Assessment Tool were also estimated. The results showed the increase of waterborne Th-232 concentration corresponded to a progressive increase of Th accumulation and total dose rate (internal and external) in the whole body of Anabas testudineus. Considering the ERICA dose rate screening value of 10 μGyh-1, the findings can be concluded the estimated of total dose rate (< 5 μGyh-1) in Anabas testudineus is in order of small magnitude. Nevertheless, these preliminary results showed that the Anabas testudineus has a potential to accumulate thorium. (author)

  17. Analysis on Forensic Identification of Family Violence in 232 Cases%232例家庭暴力损伤法医学鉴定分析

    Institute of Scientific and Technical Information of China (English)

    张鹏坤

    2006-01-01

    目的研究家庭暴力损伤的法医学特点.方法对232例家庭暴力案件资料按年龄、文化程度、职业、凶器、损伤部位、时间列表进行统计学处理.结果家庭暴力具有较强的隐蔽性的特点,多发生在家中及夜间;被鉴定人的心理较复杂、年龄多集中在26~35岁之间、小学到中专之间随着文化程度的增高鉴定的比例呈上升趋势,有职业者多于无职业者,城镇明显多于农村.结论被鉴定人的心理、年龄、文化程度、职业与法医学鉴定的关系密切,对遏止家庭暴力的发生具有重要意义.

  18. 基于C8051F040的CAN总线与RS-232通信设计%Design of communication between CAN bus and RS-232 based on C8051F040

    Institute of Scientific and Technical Information of China (English)

    盛伟荃; 曾连荪

    2014-01-01

    为了实现对CAN总线和RS-232串口双向通信需求,提出了一种基于C8051F040单片机的数据通信方案,并完成系统设计.分析了CAN总线和RS-232串口的通信特点,介绍了单片机硬件,并对软件的设计思路与流程做了详尽描述,完成功能检测.实验结果表明,该设计达到了要求.

  19. Actinide Oxidation State and O/M Ratio in Hypostoichiometric Uranium-Plutonium-Americium U0.750Pu0.246Am0.004O2-x Mixed Oxides.

    Science.gov (United States)

    Vauchy, Romain; Belin, Renaud C; Robisson, Anne-Charlotte; Lebreton, Florent; Aufore, Laurence; Scheinost, Andreas C; Martin, Philippe M

    2016-03-01

    Innovative americium-bearing uranium-plutonium mixed oxides U1-yPuyO2-x are envisioned as nuclear fuel for sodium-cooled fast neutron reactors (SFRs). The oxygen-to-metal (O/M) ratio, directly related to the oxidation state of cations, affects many of the fuel properties. Thus, a thorough knowledge of its variation with the sintering conditions is essential. The aim of this work is to follow the oxidation state of uranium, plutonium, and americium, and so the O/M ratio, in U0.750Pu0.246Am0.004O2-x samples sintered for 4 h at 2023 K in various Ar + 5% H2 + z vpm H2O (z = ∼15, ∼90, and ∼200) gas mixtures. The O/M ratios were determined by gravimetry, XAS, and XRD and evidenced a partial oxidation of the samples at room temperature. Finally, by comparing XANES and EXAFS results to that of a previous study, we demonstrate that the presence of uranium does not influence the interactions between americium and plutonium and that the differences in the O/M ratio between the investigated conditions is controlled by the reduction of plutonium. We also discuss the role of the homogeneity of cation distribution, as determined by EPMA, on the mechanisms involved in the reduction process. PMID:26907589

  20. Novel Mutations L228I and Y232H Cause Nonnucleoside Reverse Transcriptase Inhibitor Resistance in Combinational Pattern.

    Science.gov (United States)

    Zhang, Xiao-Min; Zhang, Qiwei; Wu, Hao; Lau, Terrence Chi-Kong; Liu, Xuan; Chu, Hin; Zhang, Ke; Zhou, Jie; Chen, Zhi-Wei; Jin, Dong-Yan; Zheng, Bo-Jian

    2016-09-01

    The emergence of drug resistance mutations is increasing after the implementation of highly active antiretroviral therapy. To characterize two novel mutations L228I and Y232H in the primer grip of reverse transcriptase (RT) of HIV-1 circulating recombination form 08_BC (CRF08_BC) subtype, both mutant clones were constructed to determine their impacts on viral phenotypic susceptibility and replication capacity (RC). Results showed that the novel mutation, L228I, conferred a low-level resistance to etravirine by itself. L228I in combination with Y188C displayed a high level of cross-resistance to both nevirapine (NVP) and efavirenz (EFV). The copresence of A139V and Y232H induced a moderate level of resistance to NVP and EFV. Mutations Y188C/L228I, A139V, Y232H, and A139V/Y232H reduced more than 55% of viral RC compared with that of the wild-type (WT) reference virus. Modeling study suggested that the copresence of Y188C/L228I or A139V/Y232H might induce conformational changes to RT, which might result in reduced drug susceptibility and viral RC due to abolished hydrogen bonding or complex interaction with vicinal residues. Our results demonstrated that L228I and Y232H were novel accessory nonnucleoside reverse transcriptase inhibitor resistance-related mutations and provided valuable information for clinicians to design more effective treatment to patients infected with HIV-1 subtype CRF08_BC. PMID:27067022

  1. Fission Fragment Angular Distribution of 232Th(n,f) at the CERN n_TOF Facility

    CERN Document Server

    Tarrío, D; Audouin, L; Duran, I.; Paradela, C.; Tassan-Got, L; Altstadt, S; Andrzejewski, J; Barbagallo, M; Bécares, V; Bečvář, F; Belloni, F; Berthoumieux, E; Billowes, J; Boccone, V; Bosnar, D; Brugger, M; Calviani, M; Calviño, F; Cano-Ott, D; Carrapiço, C; Cerutti, F; Chiaveri, E; Chin, M; Colonna, N; Cortés, G; Cortés-Giraldo, M A; Diakaki, M; Domingo-Pardo, C; Dzysiuk, N; Eleftheriadis, C; Ferrari, A; Fraval, K; Ganesan, S; García, A R; Giubrone, G; Gómez-Hornillos, M B; Gonçalves, I F; González-Romero, E; Griesmayer, E; Guerrero, C; Gunsing, F; Gurusamy, P; Jenkins, D G; Jericha, E; Kadi, Y; Käppeler, F; Karadimos, D; Koehler, P; Kokkoris, M; Krtička, M; Kroll, J; Langer, C; Lederer, C; Leeb, H; Losito, R; Manousos, A; Marganiec, J; Martínez, T; Massimi, C; Mastinu, P F; Mastromarco, M; Meaze, M; Mendoza, E; Mengoni, A; Milazzo, P M; Mingrone, F; Mirea, M; Mondalaers, W; Pavlik, A; Perkowski, J; Plompen, A; Praena, J; Quesada, J M; Rauscher, T; Reifarth, R; Riego, A; Roman, F; Rubbia, C; Sarmento, R; Schillebeeckx, P; Schmidt, S; Tagliente, G; Tain, J L; Tsinganis, A; Valenta, S; Vannini, G; Variale, V; Vaz, P; Ventura, A; Versaci, R; Vermeulen, M J; Vlachoudis, V; Vlastou, R; Wallner, A; Ware, T; Weigand, M; Weiß, C; Wright, T J; Žugec, P

    2014-01-01

    The angular distribution of fragments emitted in neutron-induced fission of Th-232 was measured in the white spectrum neutron beam at the n\\_TOF facility at CERN. A reaction chamber based on Parallel Plate Avalanche Counters (PPAC) was used, where the detectors and the targets have been tilted 45 degrees with respect to the neutron beam direction in order to cover the full angular range of the fission fragments. A GEANT4 simulation has been developed to study the setup efficiency. The data analysis and the preliminary results obtained for the Th-232(n,f) between fission threshold and 100 MeV are presented here.

  2. Radioactivity of Natural Nuclides (40K, 238U, 232Th, 226Ra) in Coals from Eastern Yunnan, China

    OpenAIRE

    Xin Wang; Qiyan Feng; Ruoyu Sun; Guijian Liu

    2015-01-01

    The naturally occurring primordial radionuclides in coals might exhibit high radioactivity, and can be exported to the surrounding environment during coal combustion. In this study, nine coal samples were collected from eastern Yunnan coal deposits, China, aiming at characterizing the overall radioactivity of some typical nuclides (i.e., 40K, 238U, 232Th, 226Ra) and assessing their ecological impact. The mean activity concentrations of 238U, 232Th, 40K and 226Ra are 63.86 (17.70–92.30 Bq· kg-...

  3. Prompt γ-rays from the Fast Neutron Induced Fission on 235,238U and 232Th

    Science.gov (United States)

    Lebois, M.; Wilson, J. N.; Halipré, P.; Leniau, B.; Matea, I.; Oberstedt, A.; Oberstedt, S.; Verney, D.

    Preliminary results from the first experiment using the LICORNE neutron source at the IPN Orsay are presented. Prompt fission gamma rays from fast-neutron induced fission of 238U, 232Th and 235U were detected. Thick samples of around 50 g of 238U and 232Th are used for the first part of the experiment. An ionisation chamber containing ∼ 10 mg samples of 238U and 235U to provide a fission trigger is used for the second part of the experiment. Gamma rays have been detected using 17 high efficiency BaF2 detectors and 6 LaBr3 scintillator detectors.

  4. 238 U, 232 Th and 40 K in wheat flour samples of Iraq markets

    Directory of Open Access Journals (Sweden)

    A. A.

    2014-09-01

    Full Text Available Introduction. Wheat flour is a nutritious type of food that is widely consumed by various age groups in Iraq. This study investigates the presence of long-lived gamma emitters in different type of wheat flour in Iraqi market. Materials and methods. Uranium ( 238 U, Thorium ( 232 Th and Potassium ( 40 K specific activity in (Bq/kg were measured in (12 different types of wheat flours that are available in Iraqi markets. The gamma spectrometry method with a NaI(Tl detector has been used for radiometric measurements. Also in this study we have calculated the internal hazard index, radium equivalent and absorbed dose rate in all samples. Results and discussion. It is found that the specific activity in wheat flour samples were varied from (1.086±0.0866 Bq/kg to (12.532±2.026 Bq/kg with an average (6.6025 Bq/kg for 238 U, For 232 Th From (0.126±0.066 Bq/kg to (4.298±0.388 Bq/kg with an average (1.9465Bq/kg and for 40 K from (41.842±5.875 Bq/kg to (264.729±3.843 Bq/kg with an average (133.097 Bq/kg. Also, it is found that the radium equivalent and the internal hazard index in wheat flour samples ranged from (3.4031 Bq/kg to (35.1523 Bq/kg with an average (19.6346 Bq/kg and from (0.0091 to (0.1219 with an average (0.0708 respectively. Conclusion. This study prove that the natural radioactivity and radiation hazard indices were lower than the safe.

  5. 238 U, 232 Th and 40 K in wheat flour samples of Iraq markets

    Directory of Open Access Journals (Sweden)

    Ali Abid Abojassim

    2015-05-01

    Full Text Available Introduction. Wheat flour is a nutritious type of food that is widely consumed by various age groups in Iraq. This study investigates the presence of long-lived gamma emitters in different type of wheat flour in Iraqi market. Materials and methods. Uranium (238 U, Thorium (232 Th and Potassium (40 K specific activity in (Bq/kg were measured in (12 different types of wheat flours that are available in Iraqi markets. The gamma spectrometry method with a NaI(Tl detector has been used for radiometric measurements. Also in this study we have calculated the internal hazard index, radium equivalent and absorbed dose rate in all samples. Results and discussion. It is found that the specific activity in wheat flour samples were varied from (1.086±0.0866 Bq/kg to (12.532±2.026 Bq/kg with an average (6.6025 Bq/kg for 238 U, For 232 Th From (0.126±0.066 Bq/kg to (4.298±0.388 Bq/kg with an average (1.9465Bq/kg and for 40 K from (41.842±5.875 Bq/kg to (264.729±3.843 Bq/kg with an average (133.097 Bq/kg. Also, it is found that the radium equivalent and the internal hazard index in wheat flour samples ranged from (3.4031 Bq/kg to (35.1523 Bq/kg with an average (19.6346 Bq/kg and from (0.0091 to (0.1219 with an average (0.0708 respectively. Conclusion. This study prove that the natural radioactivity and radiation hazard indices were lower than the safe.

  6. Biological characterization and next-generation genome sequencing of the unclassified Cotia virus SPAn232 (Poxviridae).

    Science.gov (United States)

    Afonso, Priscila P; Silva, Patrícia M; Schnellrath, Laila C; Jesus, Desyreé M; Hu, Jianhong; Yang, Yajie; Renne, Rolf; Attias, Marcia; Condit, Richard C; Moussatché, Nissin; Damaso, Clarissa R

    2012-05-01

    Cotia virus (COTV) SPAn232 was isolated in 1961 from sentinel mice at Cotia field station, São Paulo, Brazil. Attempts to classify COTV within a recognized genus of the Poxviridae have generated contradictory findings. Studies by different researchers suggested some similarity to myxoma virus and swinepox virus, whereas another investigation characterized COTV SPAn232 as a vaccinia virus strain. Because of the lack of consensus, we have conducted an independent biological and molecular characterization of COTV. Virus growth curves reached maximum yields at approximately 24 to 48 h and were accompanied by virus DNA replication and a characteristic early/late pattern of viral protein synthesis. Interestingly, COTV did not induce detectable cytopathic effects in BSC-40 cells until 4 days postinfection and generated viral plaques only after 8 days. We determined the complete genomic sequence of COTV by using a combination of the next-generation DNA sequencing technologies 454 and Illumina. A unique contiguous sequence of 185,139 bp containing 185 genes, including the 90 genes conserved in all chordopoxviruses, was obtained. COTV has an interesting panel of open reading frames (ORFs) related to the evasion of host defense, including two novel genes encoding C-C chemokine-like proteins, each present in duplicate copies. Phylogenetic analysis revealed the highest amino acid identity scores with Cervidpoxvirus, Capripoxvirus, Suipoxvirus, Leporipoxvirus, and Yatapoxvirus. However, COTV grouped as an independent branch within this clade, which clearly excluded its classification as an Orthopoxvirus. Therefore, our data suggest that COTV could represent a new poxvirus genus.

  7. Integral Fission Cross Section Ratios of Th232, U236 and U238 Relative to U235 in the Neutron Spectrum Produced by 23.2 MeV Deuterons Incident on a Thick Be Metal Target

    International Nuclear Information System (INIS)

    Integral neutron fission cross section ratios have been measured for Th232 /U238 , U23S/U235 and U236/U235 in the neutron field produced by bombardment of a thick Be metal target with 23.2 MeV deuterons. Validation of Th232, U236, U23S fission cross sections in a high energy neutron continuum spectrum is the object of this work. The neutron spectrum in the irradiation site has been obtained by unfolding of the neutron induced activity of eleven selected reactions. The average standard deviation between calculated activities with SAND-II unfolding code and the experimental input activities was 2.5%. Calculated values of the fission cross section ratios were obtained from, the ENDF/B-y evaluated library of cross sections and the measured spectrum. These ratios were not sensitive (<0.7%) to quite different SAND-II input spectra assumed in the low energy spectrum range (0.5 to 2. MeV). Analysis of error sources, errors propagation and their correlations was made and the correlation matrix of the experimental results was calculated. The experimental and calculated values obtained are consistent within the errors. Examination of the fissile ratios measured in other continuum neutron spectra shows a similar consistency in the spectrum produced by 7 MeV deuterons on Be. However in Cf252 and thermal U235 fission neutron spectra, a large discrepancy is found for Th232. (author)

  8. 基于EPM7192的RS232转IO接口模块的设计与实现%Design and implementation of RS232 to IO interface module based on EPM7192

    Institute of Scientific and Technical Information of China (English)

    李金猛

    2013-01-01

    This paper introduces the design method of control card including software and hardware.The core of card is EPM7192.It consists of 5 parts:power circuit,crystal circuit,232 interface circuit,IO interface circuit as well as main process circuit.The control communication interface uses RS232,The paper emphasized on the design method of mixture input which include sch and VHDL,It also emphasized on depiction the application of ISP software [2].It also realizes the software receiving control component used by VHDL,and gave out the test application in the end.%介绍了用于自动控制设备控制板卡的软硬件设计方法,该卡以EPM7192为核心,由电源电路、晶振电路、232接口电路、IO接口电路、主处理电路等5部分组成,控制通讯接口采用RS232,叙述了用混合输入实现该设计的方法[1],并用VHDL语言实现整个软件接收控制部分,最后给出了应用测试情况.

  9. 一种简单的光电隔离RS-232电平转换接口设计%A kind of simple photoelectric-isolated RS-232 voltage conversion interface design

    Institute of Scientific and Technical Information of China (English)

    王三胜; 顾彪

    2001-01-01

    A design method of a kind of practical photoelectric-isolated RS-232 voltage conversion interface is introduced .Making use of the method ,a connection circuit is designed, which does not need RS-232 voltage converter and fulfills voltage conversion by photoelectric coupler directly. At the same time, hardware connection circuit,complete communication protocols and software design of communication between MCS-51 single-chip microcomputer and PC computer are given.%介绍一种简单实用的光电隔离RS-232电平转换接口设计方法。采用该方法设计的接口电路不需要RS-232电平转换器,由光电耦合器直接完成电平转换.并给出一个MCS-51单片机与PC机通讯的硬件连接电路、完整的通讯协议和软件设计流程。

  10. Human bones obtained from routine joint replacement surgery as a tool for studies of plutonium, americium and {sup 90}Sr body-burden in general public

    Energy Technology Data Exchange (ETDEWEB)

    Mietelski, Jerzy W., E-mail: jerzy.mietelski@ifj.edu.pl [Henryk Niewodniczanski Institute of Nuclear Physics, Polish Academy of Sciences, Radzikowskiego 152, 31-342 Cracow (Poland); Golec, Edward B. [Traumatology and Orthopaedic Clinic, 5th Military Clinical Hospital and Polyclinic, Independent Public Healthcare Facility, Wroclawska 1-3, 30-901 Cracow (Poland); Orthopaedic Rehabilitation Department, Chair of Clinical Rehabilitation, Faculty of Motor of the Bronislaw Czech' s Academy of Physical Education, Cracow (Poland); Department of Physical Therapy Basics, Faculty of Physical Therapy, Administration College, Bielsko-Biala (Poland); Tomankiewicz, Ewa [Henryk Niewodniczanski Institute of Nuclear Physics, Polish Academy of Sciences, Radzikowskiego 152, 31-342 Cracow (Poland); Golec, Joanna [Orthopaedic Rehabilitation Department, Chair of Clinical Rehabilitation, Faculty of Motor of the Bronislaw Czech' s Academy of Physical Education, Cracow (Poland); Physical Therapy Department, Institute of Physical Therapy, Faculty of Heath Science, Jagiellonian University, Medical College, Cracow (Poland); Nowak, Sebastian [Traumatology and Orthopaedic Clinic, 5th Military Clinical Hospital and Polyclinic, Independent Public Healthcare Facility, Wroclawska 1-3, 30-901 Cracow (Poland); Orthopaedic Rehabilitation Department, Chair of Clinical Rehabilitation, Faculty of Motor of the Bronislaw Czech' s Academy of Physical Education, Cracow (Poland); Szczygiel, Elzbieta [Physical Therapy Department, Institute of Physical Therapy, Faculty of Heath Science, Jagiellonian University, Medical College, Cracow (Poland); Brudecki, Kamil [Henryk Niewodniczanski Institute of Nuclear Physics, Polish Academy of Sciences, Radzikowskiego 152, 31-342 Cracow (Poland)

    2011-06-15

    The paper presents a new sampling method for studying in-body radioactive contamination by bone-seeking radionuclides such as {sup 90}Sr, {sup 239+240}Pu, {sup 238}Pu, {sup 241}Am and selected gamma-emitters, in human bones. The presented results were obtained for samples retrieved from routine surgeries, namely knee or hip joints replacements with implants, performed on individuals from Southern Poland. This allowed to collect representative sets of general public samples. The applied analytical radiochemical procedure for bone matrix is described in details. Due to low concentrations of {sup 238}Pu the ratio of Pu isotopes which might be used for Pu source identification is obtained only as upper limits other then global fallout (for example Chernobyl) origin of Pu. Calculated concentrations of radioisotopes are comparable to the existing data from post-mortem studies on human bones retrieved from autopsy or exhumations. Human bones removed during knee or hip joint surgery provide a simple and ethical way for obtaining samples for plutonium, americium and {sup 90}Sr in-body contamination studies in general public. - Highlights: > Surgery for joint replacement as novel sampling method for studying in-body radioactive contamination. > Proposed way of sampling is not causing ethic doubts. > It is a convenient way of collecting human bone samples from global population. > The applied analytical radiochemical procedure for bone matrix is described in details. > The opposite patient age correlations trends were found for 90Sr (negative) and Pu, Am (positive).

  11. The recycling of the actinides neptunium, americium and curium in a fast power reactor to reduce the long term activity in a final store

    International Nuclear Information System (INIS)

    The starting point for the considerations and calculations given in this dissertation is the inevitable production of radioactive materials in the use of nuclear energy, which creates a considerable potential danger in a final store for a very long period. As one possibility of alleviating this problem, a concept for recycling the waste actinides neptunium, americium and curium was proposed. The waste actinides are separated in the reprocessing of burnt-up fuel elements and reach a further irradiation circuit. There they pass through the stages 'manufacture of irradiation elements', 'use in a fast power reactor' and reprocessing of irradiation elements' several times. In each irradiation and subsequent storage, about 17% of the waste actinides are removed by fission or by conversion into nuclides which can be reused as fuel, so that during the life of 40 years of the fast recycling reacor, the waste actinides can be reduced in mass by one half. In order to determine this mass reduction effect, a model calculation was developed, which includes the representation of the neutron physics and thermal properties of the reactor core and the storage and reprocessing of the irradiation elements. (orig./RB)

  12. Human bones obtained from routine joint replacement surgery as a tool for studies of plutonium, americium and 90Sr body-burden in general public

    International Nuclear Information System (INIS)

    The paper presents a new sampling method for studying in-body radioactive contamination by bone-seeking radionuclides such as 90Sr, 239+240Pu, 238Pu, 241Am and selected gamma-emitters, in human bones. The presented results were obtained for samples retrieved from routine surgeries, namely knee or hip joints replacements with implants, performed on individuals from Southern Poland. This allowed to collect representative sets of general public samples. The applied analytical radiochemical procedure for bone matrix is described in details. Due to low concentrations of 238Pu the ratio of Pu isotopes which might be used for Pu source identification is obtained only as upper limits other then global fallout (for example Chernobyl) origin of Pu. Calculated concentrations of radioisotopes are comparable to the existing data from post-mortem studies on human bones retrieved from autopsy or exhumations. Human bones removed during knee or hip joint surgery provide a simple and ethical way for obtaining samples for plutonium, americium and 90Sr in-body contamination studies in general public. - Highlights: → Surgery for joint replacement as novel sampling method for studying in-body radioactive contamination. → Proposed way of sampling is not causing ethic doubts. → It is a convenient way of collecting human bone samples from global population. → The applied analytical radiochemical procedure for bone matrix is described in details. → The opposite patient age correlations trends were found for 90Sr (negative) and Pu, Am (positive).

  13. The estimation of reactions of hematopoietic systems of organisms to the effect, caused by americium and plutonium, of nuclear industry workers

    Energy Technology Data Exchange (ETDEWEB)

    Gasteva, G. N.; Ivanova, T. A.; Gordeeva, A. A.; Suvorova, L. A.; Molokanov, A. A.; Badine, I.

    2004-07-01

    Object of research are the workers having in an organism radioactive substance (Am-241 and Pu-239). The purpose of work was the estimation of reaction hemopoietic systems of an organism on influence of americium and plutonium at workers of the nuclear industry. At the surveyed contingent of persons the determined effects caused by total influence Am-241 and Pu-239 are ascertained; chronic radiation disease with development, besides diffusive a pneumoscleoris and a chronic toxic-chemical radiating bronchitis, reactions of system of blood, jet hepatopathy which frequency accrued with increase doses loadings and essentially did not depend on age. In peripheral blood on the foreground jet changes act: hyperglobulia, the tendency to neutrophilus leukocytosis, monocytosis, increase ESR, decrease (reduction ?/G of factor reflecting weight and processing of defeat bronchus and pulmonary of system. Stable downstroke in number thrombocytes and reticulocytes in peripheral blood, their direct dependence on a doze of an irradiation, reflect hypoplastic a background hemogenesis, caused by long influence incorporatedin a bone and a bone brain of radioactive substances. At cytologic research punctate a bone brain jet changes which are expressed in increase of functional activity erythro-and myelopoiesiscome to light and provide compensatory reaction of peripheral blood. At histologic research of a bone brain and a bone fabric attributes of development atrophic process which is expressed in reduction of volume parenchyma a bone brain (a fatty atrophy) and dysplasia to a bone fabric are observed.

  14. Analysis of HIV antibody test results in 232 HIV/AIDS and their spouses or fixed sex partners%232例HIV/AIDS配偶/固定性伴HIV抗体检测结果分析

    Institute of Scientific and Technical Information of China (English)

    徐智贤; 王志苏; 李春梅

    2013-01-01

    Objective:To study the infection status and sexual behavior of the HIVsexual transmission among HIV/AIDS and their spouses or fixed sex partners,and provide the basis for the prevention and spread of HIV infection.Methods:HIV antibody was detected in blood samples of HIV/AIDS cases and their spouses or fixed sex partners.Results:HIV antibody test results showed that 48 positive cases were found in 232 spouses of HIV/AIDS cases,the rate of HIV infection through sexual transmission was 20.69% (48/232).Among 31 positive male spouses,the HIV transmission rate of female-to-male was 21.68% (31/143); while in 17 positive female spouses,the HIV transmission rate of male-to-female was 19.10% (17/89).(x2 =0.222,P>0.05).The transmission rate of male-female and female-male had no significant statistical difference.HIV/AIDS and their spouses or fixed sex partners were at low education level,most were junior high school and below,accounting for 84.48% (196/232); The farmers ranked the top,accounting for 78.45% (182/232); The high peak age was between 30 and 39 years old,46.12% (107/232); The condom useage rate was extremely low.The couples with infection time interval less than three months accounted for 83.33% (40/48).Conclusion:It is effective to expand the detection range,carry out timely missionary and intervention,increase condom use for blocking the HIV transmission through sexual behaviors between spouses.%目的:掌握本市HIV/AIDS配偶/固定性伴感染现状,为预防该人群HIV感染和传播提供依据.方法:对已确认的HIV/AIDS配偶/固定性伴采血进行HIV抗体检测.结果:对232例配偶进行HIV抗体检测,检出阳性48例,配偶间传播率为20.69%(48/232).男配偶检出31例,女传男的概率为21.68%(31/143);女配偶检出17例,男传女的概率为19.10%(17/89).经x2检验,x2=0.222,P>0.05.男传女和女传男的HIV传播率差异无统计学意义.HIV/AIDS配偶/固定性伴文化

  15. 50 CFR 23.2 - How do I decide if these regulations apply to my shipment or me?

    Science.gov (United States)

    2010-10-01

    ... ENDANGERED SPECIES OF WILD FAUNA AND FLORA (CITES) Introduction § 23.2 How do I decide if these regulations... a controlled environment) listed in Appendix I, II, or III of CITES (see § 23.91)? (1) YES. Continue... wildlife or plant specimen exempted from CITES (see § 23.92)? (1) YES. The regulations in this part do...

  16. U-238, Th-232, K-40 along the main 3 km adit of the Baksan Neutrino Observatory

    International Nuclear Information System (INIS)

    Results of the U-238, Th-232, K-40 contents in the mountain rock samples along 3 km adit of the Baksan Neutrino Observatory are presented. Recommendations on selection of suitable site for the low-background underground laboratory are given

  17. The first detection of the 232 GHz vibrationally excited H2O maser in Orion KL with ALMA

    CERN Document Server

    Hirota, Tomoya; Honma, Mareki

    2012-01-01

    We investigated the ALMA science verification data of Orion KL and found a spectral signature of the vibrationally excited H2O maser line at 232.68670 GHz (nu2=1, 5,5,0-6,4,3). This line has been detected in circumstellar envelopes of late-type stars so far but not in young stellar objects including Orion KL. Thus, this is the first detection of the 232 GHz vibrationally excited H2O maser in star-forming regions. The distribution of the 232 GHz maser is concentrated at the position of the radio Source I, which is remarkably different from other molecular lines. The spectrum shows a double-peak structure at the peak velocities of -2.1 and 13.3 km s-1. It appears to be consistent with the 22 GHz H2O masers and 43 GHz SiO masers observed around Source I. Thus, the 232 GHz H2O maser around Source I would be excited by the internal heating by an embedded protostar, being associated with either the root of the outflows/jets or the circumstellar disk around Source I, as traced by the 22 GHz H2O masers or 43 GHz SiO ...

  18. THE FIRST DETECTION OF THE 232 GHz VIBRATIONALLY EXCITED H2O MASER IN ORION KL WITH ALMA

    International Nuclear Information System (INIS)

    We investigated the ALMA science verification data of Orion KL and found a spectral signature of the vibrationally excited H2O maser line at 232.68670 GHz (ν2 = 1, 55,0-64,3). This line has been detected previously in circumstellar envelopes of late-type stars but not in young stellar objects such as Orion KL. Thus, this is the first detection of the 232 GHz vibrationally excited H2O maser in star-forming regions. The distribution of the 232 GHz maser is concentrated at the position of the radio Source I, which is remarkably different from other molecular lines. The spectrum shows a double-peak structure at the peak velocities of –2.1 and 13.3 km s–1. It appears to be consistent with the 22 GHz H2O masers and 43 GHz SiO masers observed around Source I. Thus, the 232 GHz H2O maser around Source I would be excited by the internal heating by an embedded protostar, being associated with either the root of the outflows/jets or the circumstellar disk around Source I, as traced by the 22 GHz H2O masers or 43 GHz SiO masers, respectively.

  19. 48 CFR 52.232-34 - Payment by Electronic Funds Transfer-Other than Central Contractor Registration.

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    2010-10-01

    ... PROVISIONS AND CONTRACT CLAUSES Text of Provisions and Clauses 52.232-34 Payment by Electronic Funds Transfer... payment. (1) All payments by the Government under this contract shall be made by electronic funds transfer... governing Federal payments through the ACH are contained in 31 CFR part 210. (d) Suspension of payment....

  20. 42 CFR 457.232 - Refunding of Federal Share of CHIP overpayments to providers and referral of allegations of waste...

    Science.gov (United States)

    2010-10-01

    ... 42 Public Health 4 2010-10-01 2010-10-01 false Refunding of Federal Share of CHIP overpayments to... Claims; Reduction of Federal Medical Payments § 457.232 Refunding of Federal Share of CHIP overpayments.... (a) Quarterly Federal payments to the States under title XXI (CHIP) of the Act are to be reduced...

  1. Criticality safety control for source term reduction in Scrubber Glovebox of Building 232-Z. CSER 90-006, Addendum 1

    International Nuclear Information System (INIS)

    This Criticality Safety Evaluation Report addendum extends the coverage of the original CSAR (90-006) about dismantling the ductwork in 232-Z to include cleanout of the Scrubber Glovebox, with an estimated residual Pu holdup of less than 200 grams. The procedures for keeping any materials inside or removed dry is retained as part of the qualification as a Limited Control Facility

  2. Measurement of fission products yields in the quasi-mono-energetic neutron-induced fission of 232Th

    Science.gov (United States)

    Naik, H.; Mukherji, Sadhana; Suryanarayana, S. V.; Jagadeesan, K. C.; Thakare, S. V.; Sharma, S. C.

    2016-08-01

    The cumulative yields of various fission products in the 232Th(n, f) reaction at average neutron energies of 5.42, 7.75, 9.35 and 12.53 MeV have been determined by using an off-line γ-ray spectrometric technique. The neutron beam was produced from the 7Li(p, n) reaction by using the proton energies of 7.8, 12, 16 and 20 MeV. The mass chain yields were obtained from the cumulative fission yields by using the charge distribution correction of medium energy fission. The fine structure in the mass yield distribution was interpreted from the point of nuclear structure effect. On the other hand, the higher yield around mass number 133-134 and 143-144 as well as their complementary products were explained based on the standard I and standard II asymmetric mode of fission. From the mass yield data, the average value of light mass (), heavy mass (), the average number of neutrons () and the peak-to-valley (P / V) ratios at different neutron energies of present work and literature data were obtained in the 232Th(n, f) reaction. The different parameters of the mass yield distribution in the 232Th(n, f) reaction were compared with the similar data in the 232Th(γ, f) reaction at comparable excitation energy and a surprising difference was observed.

  3. The reductive half-reaction of xanthine dehydrogenase from Rhodobacter capsulatus: the role of Glu232 in catalysis.

    Science.gov (United States)

    Hall, James; Reschke, Stefan; Cao, Hongnan; Leimkühler, Silke; Hille, Russ

    2014-11-14

    The kinetic properties of an E232Q variant of the xanthine dehydrogenase from Rhodobacter capsulatus have been examined to ascertain whether Glu(232) in wild-type enzyme is protonated or unprotonated in the course of catalysis at neutral pH. We find that kred, the limiting rate constant for reduction at high [xanthine], is significantly compromised in the variant, a result that is inconsistent with Glu(232) being neutral in the active site of the wild-type enzyme. A comparison of the pH dependence of both kred and kred/Kd from reductive half-reaction experiments between wild-type and enzyme and the E232Q variant suggests that the ionized Glu(232) of wild-type enzyme plays an important role in catalysis by discriminating against the monoanionic form of substrate, effectively increasing the pKa of substrate by two pH units and ensuring that at physiological pH the neutral form of substrate predominates in the Michaelis complex. A kinetic isotope study of the wild-type R. capsulatus enzyme indicates that, as previously determined for the bovine and chicken enzymes, product release is principally rate-limiting in catalysis. The disparity in rate constants for the chemical step of the reaction and product release, however, is not as great in the bacterial enzyme as compared with the vertebrate forms. The results indicate that the bacterial and bovine enzymes catalyze the chemical step of the reaction to the same degree and that the faster turnover observed with the bacterial enzyme is due to a faster rate constant for product release than is seen with the vertebrate enzyme.

  4. Gastric cancer at a university teaching hospital in northwestern Tanzania: a retrospective review of 232 cases

    Directory of Open Access Journals (Sweden)

    Mabula Joseph B

    2012-11-01

    Full Text Available Abstract Background Despite marked decreases in its incidence, particularly in developed countries, gastric cancer is still the second most common tumor worldwide. There is a paucity of information regarding gastric cancer in northwestern Tanzania. This study was undertaken to describe our experience, in our local setting, on the management of gastric cancer, outlining the clinicopathological and treatment outcome of these patients and suggesting ways to improve the treatment outcome. Methods This was a retrospective study of histologically confirmed cases of gastric cancer seen at Bugando Medical Centre between January 2007 and December 2011. Data were retrieved from patients’ files and analyzed using SPSS computer software version 17.0. Results A total of 232 gastric cancer patients were enrolled in the study, representing 4.5% of all malignancies. The male to female ratio was 2.9:1. The median age of patients was 52 years. The majority of the patients (92.1% presented late with advanced gastric cancer (Stages III and IV. Lymph node and distant metastasis at the time of diagnosis was recorded in 31.9% and 29.3% of cases, respectively. The antrum was the most frequent anatomical site (56.5% involved and gastric adenocarcinoma (95.1% was the most common histopathological type. Out of 232 patients, 223 (96.1% patients underwent surgical procedures for gastric cancer of which gastro-jejunostomy was the most frequent performed surgical procedure, accounting for 53.8% of cases. The use of chemotherapy and radiotherapy was documented in 56 (24.1% and 12 (5.1% patients, respectively. Postoperative complication and mortality rates were 37.1% and 18.1%, respectively. According to multivariate logistic regression analysis, preoperative co-morbidity, histological grade and stage of the tumor, presence of metastases at the time of diagnosis was the main predictors of death (P P Conclusions Gastric cancer in this region shows a trend towards relative

  5. Infarctions in the vascular territory of the posterior cerebral artery: clinical features in 232 patients

    Directory of Open Access Journals (Sweden)

    Parra Olga

    2011-09-01

    Full Text Available Abstract Background Ischemic stroke caused by infarction in the territory of the posterior cerebral artery (PCA has not been studied as extensively as infarctions in other vascular territories. This single centre, retrospective clinical study was conducted a to describe salient characteristics of stroke patients with PCA infarction, b to compare data of these patients with those with ischaemic stroke due to middle cerebral artery (MCA and anterior cerebral artery (ACA infarctions, and c to identify predictors of PCA stroke. Findings A total of 232 patients with PCA stroke were included in the "Sagrat Cor Hospital of Barcelona Stroke Registry" during a period of 19 years (1986-2004. Data from stroke patients are entered in the stroke registry following a standardized protocol with 161 items regarding demographics, risk factors, clinical features, laboratory and neuroimaging data, complications and outcome. The characteristics of these 232 patients with PCA stroke were compared with those of the 1355 patients with MCA infarctions and 51 patients with ACA infarctions included in the registry. Infarctions of the PCA accounted for 6.8% of all cases of stroke (n = 3808 and 9.6% of cerebral infarctions (n = 2704. Lacunar infarction was the most frequent stroke subtype (34.5% followed by atherothrombotic infarction (29.3% and cardioembolic infarction (21.6%. In-hospital mortality was 3.9% (n = 9. Forty-five patients (19.4% were symptom-free at hospital discharge. Hemianopia (odds ratio [OR] = 6.43, lacunar stroke subtype (OR = 2.18, symptom-free at discharge (OR = 1.92, limb weakness (OR = 0.10, speech disorders (OR = 0.33 and cardioembolism (OR = 0.65 were independent variables of PCA stroke in comparison with MCA infarction, whereas sensory deficit (OR = 2.36, limb weakness (OR = 0.11 and cardioembolism as stroke mechanism (OR = 0.43 were independent variables associated with PCA stroke in comparison with ACA infarction. Conclusions Lacunar stroke is

  6. The construction of TRIGA-TRAP and direct high-precision Penning trap mass measurements on rare-earth elements and americium

    Energy Technology Data Exchange (ETDEWEB)

    Ketelaer, Jens

    2010-06-14

    The construction of TRIGA-TRAP and direct high-precision Penning trap mass measurements on rare-earth elements and americium: Nuclear masses are an important quantity to study nuclear structure since they reflect the sum of all nucleonic interactions. Many experimental possibilities exist to precisely measure masses, out of which the Penning trap is the tool to reach the highest precision. Moreover, absolute mass measurements can be performed using carbon, the atomic-mass standard, as a reference. The new double-Penning trap mass spectrometer TRIGA-TRAP has been installed and commissioned within this thesis work, which is the very first experimental setup of this kind located at a nuclear reactor. New technical developments have been carried out such as a reliable non-resonant laser ablation ion source for the production of carbon cluster ions and are still continued, like a non-destructive ion detection technique for single-ion measurements. Neutron-rich fission products will be available by the reactor that are important for nuclear astrophysics, especially the r-process. Prior to the on-line coupling to the reactor, TRIGA-TRAP already performed off-line mass measurements on stable and long-lived isotopes and will continue this program. The main focus within this thesis was on certain rare-earth nuclides in the well-established region of deformation around N {proportional_to} 90. Another field of interest are mass measurements on actinoids to test mass models and to provide direct links to the mass standard. Within this thesis, the mass of {sup 241}Am could be measured directly for the first time. (orig.)

  7. Experience gained during remedial action at residential properties contaminated with Th-232 and Ra-226

    International Nuclear Information System (INIS)

    Seventeen residential properties contaminated with Th-232 and Ra-226 were decontaminated and restored by Bechtel National, Inc., during 1984 as part of the US Department of Energy's Formerly Utilized Sites Remedial Action Program. The extent of contamination varied from only a few cubic yards of material in the edge of one lawn to extensive contamination around foundations and under basement floors. Three unusual case histories will be described in detail. In the first case, a few cubic yards of contamination were expected, but more than 100 cubic yards were found. In Case 2, contamination was found under the floor of an addition to a house. Case 3 involved a home built on a lot where contaminated soils had been used as fill material to depths of up to 10 feet. The remedial action included the removal of the basement, including the floor slab and foundation. This paper will provide details about several lessons learned during remedial action at residential properties: (a) radiological characterization surveys must be thorough; (b) interviews with owners can provide helpful information about unusual or unexpected contamination problems; (c) radiological monitoring during construction is necessary for efficient and thorough remedial action; and (d) good public relations are an important element of residential remedial action projects. While these lessons may seem to be common sense items, the circumstances that require their use are often very subtle. As the case histories show, successful remedial action requires constant vigilance and careful attention to details

  8. Measurement of the 232thorium capture cross section at n-TOF-CERN

    International Nuclear Information System (INIS)

    Within the context of nuclear power as a sustainable energy resource, a program of research is concentrated on a new nuclear fuel cycle based on thorium. The main advantage, as compared to the uranium cycle, is a lower production of minor actinides, of which the radiological impact on the long term constitutes a problem. At present, nuclear data libraries don't provide cross sections of a good enough quality, allowing more realistic calculations from simulations related to these reactors. The 232Th neutron capture cross section is an example. With the n-TOF collaboration, the measurement of this reaction was achieved in 2002 using two C6D6 detectors. The experimental area located at CERN, is characterized by an outstanding neutron energy resolution coupled to a high instantaneous neutron flux. The determination of the gamma-ray cascade detection efficiency, with a random behaviour, has been obtained by the use of weighting functions. These were deduced from Monte Carlo simulations with the code MCNP. Data extraction, reduction, and the description of the neutron flux have lead to the capture yield. In the resolved resonance region, the resonance parameters describing the cross section were deduced with the code SAMMY, using the R-matrix theory. In the unresolved resonance region, an uncertainty of 3,5% is found, and a comparison with recent measurements shows a good agreement. (author)

  9. Study of the violent collisions between 63Cu+232Th at 35 MeV/nucleon

    Science.gov (United States)

    Cibor, J.; Majka, Z.; Kozik, T.; Staszel, P.; Sosin, Z.; Hagel, K.; Li, J.; Lou, L.; Tezkratt, R.; Utley, D.; Wada, R.; Xiao, B.; Natowitz, J. B.

    1997-01-01

    A study of the decay of hot and heavy composite nuclei produced in the violent collisions between 63Cu and 232Th at 35A MeV is presented. The measurement of fission fragment correlations indicates that ~ 70% of the projectile linear momentum can be transferred to the fissioning system. Heavy reaction products were observed at a laboratory angle of θ=6° in coincidence with neutrons, light charged particles, and intermediate mass fragments. The dynamical aspects of the collisions between the projectile and target nuclei were investigated using the computer code CHIMERA which is based upon the molecular dynamics concept. Asymptotic characteristics of the reaction products were confronted with results of calculations of the tandem CHIMERA plus GEMINI codes. The data and model comparisons show that a composite system of mass as high as 275 amu and with an excitation energy ~ 1 GeV is formed in the most violent collisions. Some of the heavy reaction remnants are located on the fragment mass versus velocity plane inside the area where the evaporation residues resulting from the decay of the hot composite system are expected. A high neutron multiplicity associated with these events indicates their origin in the most dissipative events. However, a low cross section for the production of these remnants and the close similarity of their characteristics to the fission fragments do not allow more conclusive statements.

  10. Analysis of 232 total fertilization failure cycles during intracytoplasmic sperm injection

    Directory of Open Access Journals (Sweden)

    Esma Sarikaya

    2011-01-01

    Full Text Available Background: The intracytoplasmic sperm injection procedure ending with total fertilization failure is very distressfull event for both the clinician and the patient.Objective: The aim of this study was to identify independent factors which could be used to identify total fertilization failure before the day of intracytoplasmic sperm injection.Materials and Methods: This was a retrospective study of 232 patients who were admitted to a tertiary-care hospital IVF Unit and showed total fertilization failure during intracytoplasmic sperm injection cycles. To sort out the interwined effects of female age, basal FSH, sperm quality, antral follicle count, starting dose of gonadotrophine, sperm extraction technique, cycle length, >14 mm follicle number, oocyte number after oocyte pick up, estradiol and progesterone level on the day of hCG and the MI, MII and GV oocyte number on the fertilization, multiple logistic regression analysis was used.Results: The total fertilization failure rate was 6% and the recurrance rate was 23%. The original model illustrated that the presence of GV oocytes, total oocyte number less than six, <2000 pg/mL E2 concentration on the day of hCG and testicular sperm extraction increases the total fertilization failure risk.Conclusion: It is very difficult to predict total fertilization failure. Sometimes even with one good quality oocyte and sperm and in the case of globozoospermia fertilization can be achieved. Not only azoospermia but also low oocyte numbers increase the chance of total fertilization failure even after intracytoplasmic sperm injection

  11. Transfer reaction cross sections from the interactions of 20Ne and 22Ne with 232Th

    International Nuclear Information System (INIS)

    A target of 232Th has been bombarded with 114 MeV 22Ne and with 114 MeV and 129 MeV 20Ne beams. Recoiling reaction products were chemically isolated and the cross sections for protactinium, uranium, and neptunium isotopes were determined. The width of the cross section distributions for a given Z and their neutron-richness are the same as those for similar transfers in Ne+ 248Cm reactions. Population of low spin isomeric states is favored in these reactions over population of high spin states. As was seen in reactions with heavier targets, an increase in reaction energy does little to shift the evaporation residues toward neutron deficiency. The implications are that only primary products with little or no excitation energy and angular momentum survive the fission process to become evaporation residues in these systems, and that the production of these nuclides is more controlled by the change in the identity of the projectile than by the corresponding change in the target

  12. Two-photon laser excitation of trapped 232Th+ ions via the 402 nm resonance line

    CERN Document Server

    Herrera-Sancho, O A; Zimmermann, K; Tamm, Chr; Peik, E; Taichenachev, A V; Yudin, V I; Glowacki, P

    2012-01-01

    Experiments on one- and two-photon laser excitation of 232Th+ ions in a radiofrequency ion trap are reported. As the first excitation step, the strongest resonance line at 402 nm from the 6d^2 7s J=3/2 ground state to the 6d7s7p J=5/2 state at 24874 cm^{-1} is driven by radiation from an extended cavity diode laser. Spontaneous decay of the intermediate state populates a number of low-lying metastable states, thus limiting the excited state population and fluorescence signal obtainable with continuous laser excitation. We study the collisional quenching efficiency of helium, argon, and nitrogen buffer gases, and the effect of repumping laser excitation from the three lowest-lying metastable levels. The experimental results are compared with a four-level rate equation model, that allows us to deduce quenching rates for these buffer gases. Using laser radiation at 399 nm for the second step, we demonstrate two-photon excitation to the state at 49960 cm^{-1}, among the highest-lying classified levels of Th+. Thi...

  13. 6,6 '-bis (5,5,8,8-tetramethyl-5,6,7,8-tetra-hydro-benzo 1,2,4 triazine-3-yl) 2,2 ' bipyridine, an effective extracting agent for the separation of americium(III) and curium(III) from the lanthanides

    International Nuclear Information System (INIS)

    The extraction of americium(III), curium(III), and the lanthanides(III) from nitric acid by 6,6'- bis (5,5,8,8-tetramethyl-5,6,7,8-tetra-hydro-benzo[1,2,4]triazine-3-yl)-[2,2'] bipyridine (CyMe4-BTBP) has been studied. Since the extraction kinetics were slow, N,N'-dimethyl-N,N'-di-octyl-2-(2-hexyl-oxy-ethyl)malonamide (DMDOHEMA) was added as a phase transfer reagent. With a mixture of 0.01 M CyMe4-BTBP + 0.25 M DMDOHEMA in n -octanol, extraction equilibrium was reached within 5 min of mixing. At a nitric acid concentration of 1 M, an americium(III) distribution ratio of approx. 10 was achieved. Americium(III)/lanthanide(III) separation factors between 50 (dysprosium) and 1500 (lanthanum) were obtained. Whereas americium(III) and curium(III) were extracted as di-solvates, the stoichiometries of the lanthanide(III) complexes were not identified unambiguously, owing to the presence of DMDOHEMA. In the absence of DMDOHEMA, both americium(III) and europium(III) were extracted as di-solvates. Back-extraction with 0.1 M nitric acid was thermodynamically possible but rather slow. Using a buffered glycolate solution of pH=4, an americium(III) distribution ratio of 0.01 was obtained within 5 min of mixing. There was no evidence of degradation of the extractant, for example, the extraction performance of CyMe4-BTBP during hydrolysis with 1 M nitric acid did not change over a two month contact. (authors)

  14. Design of high-speed portable RS 232/422 signal simulator%高速便携式RS 232/422信号模拟器设计

    Institute of Scientific and Technical Information of China (English)

    2013-01-01

    For the need of out⁃field troubleshooting for airborne flight test equipments or instrumentations,a high⁃speed por⁃table simulator which can simulate various aircraft’s RS 232/422 bus signals is designed based on FPGA and USB interface tech⁃nology. The signal simulator could generate 24 kinds of standard or nonstandard baud rate signals,it has USB interface,key⁃board and LED panel,and has the characteristics of easy setting,flexible operating,high reliability and low power consumption.%  为了飞行试验中机载测试设备或仪器外场排故的需要,利用FPGA和USB接口技术成功设计了可模拟当前各种飞机RS 232/422总线信号的高速便携式模拟器。该信号模拟器能产生24种标准或者非标准波特率的RS 232/422信号,拥有USB接口、键盘和LED显示屏等功能,具有设置简便,使用灵活,可靠性高以及耗电量低等特点。

  15. Soil-to-root vegetable transfer factors for 226Ra, 232Th, 40K, and 88Y in Malaysia

    International Nuclear Information System (INIS)

    Soil-to-plant transfer factors (TFs) are of fundamental importance in assessing the environmental impact due to the presence of radioactivity in soil and agricultural crops. Tapioca and sweet potato, both root crops, are popular foodstuffs for a significant fraction of the Malaysian population, and result in intake of radionuclides. For the natural field conditions experienced in production of these foodstuffs, TFs and the annual effective dose were evaluated for the natural radionuclides 226Ra, 232Th, 40K, and for the anthropogenic radionuclide 88Y, the latter being a component of fallout. An experimental tapioca field was developed for study of the time dependence of plant uptake. For soil samples from all study locations other than the experimental field, it has been shown that these contain the artificial radionuclide 88Y, although the uptake of 88Y has only been observed in the roots of the plant Manihot esculenta (from which tapioca is derived) grown in mining soil. The estimated TFs for 226Ra and 232Th for tapioca and sweet potato are very much higher than that reported by the IAEA. For all study areas, the annual effective dose from ingestion of tapioca and sweet potato are estimated to be lower than the world average (290 μSv y−1). - Highlights: • Transfer factors of 226Ra, 232Th, 40K, and 88Y radionuclides were estimated for widely consumed root vegetables in Malaysia. • An experimental tapioca field was developed for study of the time dependence of plant uptakes. • The estimated TF values of 226Ra and 232Th for tapioca and sweet potato are higher than the IAEA reported values. • These site-specific TFs are of importance for model derivations for tropical regions

  16. Defense In-Depth Accident Analysis Evaluation of Tritium Facility Bldgs. 232-H, 233-H, and 234-H

    International Nuclear Information System (INIS)

    'The primary purpose of this report is to document a Defense-in-Depth (DID) accident analysis evaluation for Department of Energy (DOE) Savannah River Site (SRS) Tritium Facility Buildings 232-H, 233-H, and 234-H. The purpose of a DID evaluation is to provide a more realistic view of facility radiological risks to the offsite public than the bounding deterministic analysis documented in the Safety Analysis Report, which credits only Safety Class items in the offsite dose evaluation.'

  17. Determination of 228Th, 232Th, and228Ra in wild mushroom from a naturally high radioactive region in Brazil

    International Nuclear Information System (INIS)

    Mushrooms are fungi which efficiently accumulate radionuclides, as verified by radiochemistry analyses of specimens collected in contaminated areas, specifically after the Chernobyl nuclear accident. Many studies have demonstrated that mushrooms can be used in monitoring of ecosystem contamination and quality. The present paper is part of a broader study conducted in the Pocos de Caldas plateau region in Minas Gerais, Brazil, investigating assimilation of natural Uranium and Thorium radionuclide series by mushrooms. This region has elevated natural radioactivity due to the presence of radiological anomalies of volcanic origin. These anomalies are ore bodies containing Uranium and Thorium, the later being highly predominant. Many researchers have been conducted concerning radionuclide incorporation by agricultural products on the plateau. The present paper aims to determine 232Th, 228Th, and 228Ra radionuclides in wild mushrooms collected at different locations in the plateau region. 228Ra was determined by radiochemical separation using sulphate coprecipitation followed by beta radiometry. 232Th and 228Th were determined using anion exchange resin purification followed by alpha spectrometry. Higher values were obtained to 228Th than to 232Th. This is due to higher 228Ra mobility, which decays to 228Th. The accuracy of the analytical methods employed was evaluated using the reference sample IAEA Soil 327. These methods had high chemical recovery and high sensitivity. It was possible to confirm that mushrooms accumulate radionuclide and so can be used in environmental contamination and quality assessment. (author)

  18. [About the contents of 40K, 226Ra and 232Th in forest soils of the Republic of Belarus].

    Science.gov (United States)

    Perevolotskiĭ, A N; Perevolotskaia, T V

    2014-01-01

    The specific activity of 40K, 232Th and 226Ra in forest soil ecotopes (A2-B2-C2-D2) has been investigated. When the fertility of the soil increases from A2 to D2, then the specific activity of 40K increases in the rooting zone of the soil from 275 ± 6.9 up to 499 ± 11 Bq/kg, 232Th--from 11.8 ± 0.5 to 17.1 ± 1.1 Bq/kg, 226Ra- from 19.2 γ 0.8 to 27.9 ± 1.5 Bq/kg. The calculated capacity of the absorbed dose of γ-radiation conditioned by 40K, 232Th and 226Ra increases from A2 to D2 from 27.5 ± 0.5 to 44.1 ± 1.1 nGy / h at the height of 1 m.

  19. Corrective Action Investigation Plan for Corrective Action Unit 232: Area 25 Sewage Lagoons, Nevada Test Site, Nevada, Revision 0

    International Nuclear Information System (INIS)

    The Corrective Action Investigation Plan for Corrective Action Unit 232, Area 25 Sewage Lagoons, has been developed in accordance with the Federal Facility Agreement and Consent Order that was agreed to by the U.S. Department of Energy, Nevada Operations Office; the State of Nevada Division of Environmental Protection; and the U. S. Department of Defense. Corrective Action Unit 232 consists of Corrective Action Site 25-03-01, Sewage Lagoon. Corrective Action Unit 232, Area 25 Sewage Lagoons, received sanitary effluent from four buildings within the Test Cell ''C'' Facility from the mid-1960s through approximately 1996. The Test Cell ''C'' Facility was used to develop nuclear propulsion technology by conducting nuclear test reactor studies. Based on the site history collected to support the Data Quality Objectives process, contaminants of potential concern include volatile organic compounds, semivolatile organic compounds, Resource Conservation and Recovery Act metals, petroleum hydrocarbons, polychlorinated biphenyls, pesticides, herbicides, gamma emitting radionuclides, isotopic plutonium, isotopic uranium, and strontium-90. A detailed conceptual site model is presented in Section 3.0 and Appendix A of this Corrective Action Investigation Plan. The conceptual model serves as the basis for the sampling strategy. Under the Federal Facility Agreement and Consent Order, the Corrective Action Investigation Plan will be submitted to the Nevada Division of Environmental Protection for approval. Field work will be conducted following approval of the plan. The results of the field investigation will support a defensible evaluation of corrective action alternatives in the Corrective Action Decision Document

  20. Transfer of Radionuclides K-40, Th-232 and Ra-226 from Mining Soil to Sawi (Japanese Mustard)

    Science.gov (United States)

    Hariandra, M.; Amin, Y. M.

    2008-05-01

    The uptake of naturally occurring thorium, radium and potassium by sawi (Japanese Mustard) from disused tin mining was studied. Both soil and sawi sample were collected from a vegetable farm located 15 km from Kuala Lumpur, Malaysia where the farm has been operating for 22 years on a disused tin mining. By using a gamma spectroscopy system, the transfers of radionuclides from soil to plants were investigated. The highest values of radionuclides in the soil was K-40 which is 52.8 Bq kg-1 and the lowest was Ra-226 which is 6.51 Bq kg-1. The activity of Th-232 is 18.5 Bq kg-1. The activity of radionuclides in the sawi sample shows higher values as compared to the soil sample. The highest values of radionuclides in the sawi were K-40 which is 446 Bq kg-1 and the lowest was Ra-226 which is 17.5 Bq kg-1. The activity of Th-232 is 65.2 Bq kg-1. The concentration of radionuclides in soils and plants can be used for the determination of soil-to-plant transfer factors. The soil to plant transfer factors (TF) were calculated and observed to be 2.68 for radium-226, 3.52 for thorium-232 and the highest which is 3.97 for potassium-40.

  1. Fission fragments mass distributions of nuclei populated by the multinucleon transfer channels of the 18O + 232Th reaction

    Science.gov (United States)

    Léguillon, R.; Nishio, K.; Hirose, K.; Makii, H.; Nishinaka, I.; Orlandi, R.; Tsukada, K.; Smallcombe, J.; Chiba, S.; Aritomo, Y.; Ohtsuki, T.; Tatsuzawa, R.; Takaki, N.; Tamura, N.; Goto, S.; Tsekhanovich, I.; Petrache, C. M.; Andreyev, A. N.

    2016-10-01

    It is shown that the multinucleon transfer reactions is a powerful tool to study fission of exotic neutron-rich actinide nuclei, which cannot be accessed by particle-capture or heavy-ion fusion reactions. In this work, multinucleon transfer channels of the 18O + 232Th reaction are used to study fission of fourteen nuclei 231,232,233,234Th, 232,233,234,235,236Pa, and 234,235,236,237,238U. Identification of fissioning nuclei and of their excitation energy is performed on an event-by-event basis, through the measurement of outgoing ejectile particle in coincidence with fission fragments. Fission fragment mass distributions are measured for each transfer channel, in selected bins of excitation energy. In particular, the mass distributions of 231,234Th and 234,235,236Pa are measured for the first time. Predominantly asymmetric fission is observed at low excitation energies for all studied cases, with a gradual increase of the symmetric mode towards higher excitation energy. The experimental distributions are found to be in general agreement with predictions of the fluctuation-dissipation model.

  2. 8Dim calculations of the third barrier in $^{232}$Th and a conflict between theory and experiment on uranium nuclei

    CERN Document Server

    Jachimowicz, P; Skalski, J

    2013-01-01

    We find the height of the third fission barrier $B_{III}$ and energy of the third minimum $E_{III}$ in $^{232}$Th using the macroscopic - microscopic model, very well tested in this region of nuclei. For the first time it is done on an 8-dimensional deformation hypercube. The dipole distortion is included among the shape variables to assure that no important shapes are missed. The saddle point is found on a lattice containing more than 50 million points by the immersion water flow (IWF) method. The shallow third minimum, $B_{III}-E_{III}\\approx 0.36$ MeV, agrees with experimetal data of Blons et al. This is in a sharp contrast with the status of the IIIrd minima in $^{232-236}$U: their experimental depth of $\\geq3$ MeV contradicts all realistic theoretical predictions. We emphasize the importance of repeating the experiment on $^{232}$Th, by a technique similar to that used in the uranium nuclei, for settling the puzzle of the third minima in actinides.

  3. Production of Actinium-225 via High Energy Proton Induced Spallation of Thorium-232

    International Nuclear Information System (INIS)

    The science of cancer research is currently expanding its use of alpha particle emitting radioisotopes. Coupled with the discovery and proliferation of molecular species that seek out and attach to tumors, new therapy and diagnostics are being developed to enhance the treatment of cancer and other diseases. This latest technology is commonly referred to as Alpha Immunotherapy (AIT). Actinium-225/Bismuth-213 is a parent/daughter alpha-emitting radioisotope pair that is highly sought after because of the potential for treating numerous diseases and its ability to be chemically compatible with many known and widely used carrier molecules (such as monoclonal antibodies and proteins/peptides). Unfortunately, the worldwide supply of actinium-225 is limited to about 1,000mCi annually and most of that is currently spoken for, thus limiting the ability of this radioisotope pair to enter into research and subsequently clinical trials. The route proposed herein utilizes high energy protons to produce actinium-225 via spallation of a thorium-232 target. As part of previous R and D efforts carried out at Argonne National Laboratory recently in support of the proposed US FRIB facility, it was shown that a very effective production mechanism for actinium-225 is spallation of thorium-232 by high energy proton beams. The base-line simulation for the production rate of actinium-225 by this reaction mechanism is 8E12 atoms per second at 200 MeV proton beam energy with 50 g/cm2 thorium target and 100 kW beam power. An irradiation of one actinium-225 half-life (10 days) produces ∼100 Ci of actinium-225. For a given beam current the reaction cross section increases slightly with energy to about 400 MeV and then decreases slightly for beam energies in the several GeV regime. The object of this effort is to refine the simulations at proton beam energies of 400 MeV and above up to about 8 GeV. Once completed, the simulations will be experimentally verified using 400 MeV and 8 GeV protons

  4. Production of Actinium-225 via High Energy Proton Induced Spallation of Thorium-232

    Energy Technology Data Exchange (ETDEWEB)

    Harvey, James T.; Nolen, Jerry; Vandergrift, George; Gomes, Itacil; Kroc, Tom; Horwitz, Phil; McAlister, Dan; Bowers, Del; Sullivan, Vivian; Greene, John

    2011-12-30

    The science of cancer research is currently expanding its use of alpha particle emitting radioisotopes. Coupled with the discovery and proliferation of molecular species that seek out and attach to tumors, new therapy and diagnostics are being developed to enhance the treatment of cancer and other diseases. This latest technology is commonly referred to as Alpha Immunotherapy (AIT). Actinium-225/Bismuth-213 is a parent/daughter alpha-emitting radioisotope pair that is highly sought after because of the potential for treating numerous diseases and its ability to be chemically compatible with many known and widely used carrier molecules (such as monoclonal antibodies and proteins/peptides). Unfortunately, the worldwide supply of actinium-225 is limited to about 1,000mCi annually and most of that is currently spoken for, thus limiting the ability of this radioisotope pair to enter into research and subsequently clinical trials. The route proposed herein utilizes high energy protons to produce actinium-225 via spallation of a thorium-232 target. As part of previous R and D efforts carried out at Argonne National Laboratory recently in support of the proposed US FRIB facility, it was shown that a very effective production mechanism for actinium-225 is spallation of thorium-232 by high energy proton beams. The base-line simulation for the production rate of actinium-225 by this reaction mechanism is 8E12 atoms per second at 200 MeV proton beam energy with 50 g/cm2 thorium target and 100 kW beam power. An irradiation of one actinium-225 half-life (10 days) produces {approx}100 Ci of actinium-225. For a given beam current the reaction cross section increases slightly with energy to about 400 MeV and then decreases slightly for beam energies in the several GeV regime. The object of this effort is to refine the simulations at proton beam energies of 400 MeV and above up to about 8 GeV. Once completed, the simulations will be experimentally verified using 400 MeV and 8 Ge

  5. 武汉市空气中~(238)U、~(226)Ra、~(232)Th放射性浓度估算

    Institute of Scientific and Technical Information of China (English)

    施锦华; 陈昌华

    1989-01-01

    本文报道武汉市空气中~(238)U、~(226)Ra、~(232)Th 放射性浓度的估算结果。空气中~(238)U、~(226)Ra、~(232)Th 的放射性浓度是根据地面空气中铀、镭、钍的主要天然来源是土壤粒子的再悬浮的假定,通过调查测量武汉市土壤中天然放射性核素含量和空气中含尘量,经计算后确定的。我们于1984年4—10月在武汉地区采集了60个土壤样品,调查测量了土壤中天然放射性核素含量,并根据在1981—1985年间采集的7346个空气粉尘样品测得的空气中含尘量,估算出武汉市空气中~(238)U、~(226)Ra 和~(232)Th 放射性浓度的五年平均值分别为24.0、18.9和28.7nBq/L。五年中以1983年的平均值最高,分别为30.4、23.9和36.2nBq/L。以1984和1985年的数据为例,空气中~(238)U、(226)Ra、~(232)Th 放射性浓度呈明显的季节性变化,两年中均以冬季为最高,夏季最低。在武汉市六个城区中,空气中~(238)U、~(226)Ra、~(232)Th 的放射性浓度,以青山区最高,武昌区最低。

  6. Two new cases with microdeletion of 17q23.2 suggest presence of a candidate gene for sensorineural hearing loss within this region

    DEFF Research Database (Denmark)

    Schönewolf-Greulich, Bitten; Ronan, Anne; Ravn, Kristine;

    2011-01-01

    . In this report, we describe two new 17q23.2 deletion patients with mild intellectual disability and sensorineural hearing loss. They both had submicroscopic deletions smaller than the common deleted region for the 8 previously described 17q23.2 microdeletion cases. TBX4 was previously suggested...... as the responsible gene for the heart or limb defects observed in 17q23.2 deletion patients, but the present cases do not have these features despite deletion of this gene. The finding of sensorineural hearing loss in 5 of the 10 cases, including the present cases, with a microdeletion at17q23.2, strongly suggests...... the presence of a candidate gene for hearing loss within this region. We screened 41 patients with profound sensorineural hearing loss for mutations of TBX2 and detected no mutations....

  7. Impact of the cation distribution homogeneity on the americium oxidation state in the U0.54Pu0.45Am0.01O2-x mixed oxide

    Science.gov (United States)

    Vauchy, Romain; Robisson, Anne-Charlotte; Martin, Philippe M.; Belin, Renaud C.; Aufore, Laurence; Scheinost, Andreas C.; Hodaj, Fiqiri

    2015-01-01

    The impact of the cation distribution homogeneity of the U0.54Pu0.45Am0.01O2-x mixed oxide on the americium oxidation state was studied by coupling X-ray diffraction (XRD), electron probe micro analysis (EPMA) and X-ray absorption spectroscopy (XAS). Oxygen-hypostoichiometric Am-bearing uranium-plutonium mixed oxide pellets were fabricated by two different co-milling based processes in order to obtain different cation distribution homogeneities. The americium was generated from β- decay of 241Pu. The XRD analysis of the obtained compounds did not reveal any structural difference between the samples. EPMA, however, revealed a high homogeneity in the cation distribution for one sample, and substantial heterogeneity of the U-Pu (so Am) distribution for the other. The difference in cation distribution was linked to a difference in Am chemistry as investigated by XAS, with Am being present at mixed +III/+IV oxidation state in the heterogeneous compound, whereas only Am(IV) was observed in the homogeneous compound. Previously reported discrepancies on Am oxidation states can hence be explained by cation distribution homogeneity effects.

  8. Dietary 232Th and 238U intakes for Japanese as obtained in a market basket study and contributions of imported foods to internal doses

    International Nuclear Information System (INIS)

    Thorium-232 and 238U contents in four food groups were measured by inductively coupled plasma mass spectrometry (ICP-MS). Daily intakes of 232Th and 238U for Japanese were estimated to 2.22 mBq and 15.5 mBq per person, respectively. Furthermore, preliminary estimations were made for the effects of imported foods on internal exposures for Japanese. (author). 16 refs., 1 fig., 3 tabs

  9. Fabrication of targets for transmutation of americium : synthesis of inertial matrix by sol-gel method. Procedure study on the infiltration of a radioactive solutions

    International Nuclear Information System (INIS)

    addition a new and unexpected phase formed by the reaction of americium with spinel during the high temperature synthesis process has been identified. This new phase could provide a unique menas to stabilise Am in one particular oxidation state. (Author)

  10. Sorption and diffusion of cobalt, nickel, strontium, iodine, cesium and americium in natural fissure surfaces and drill core cups studied by autoradiography, 3

    International Nuclear Information System (INIS)

    This report summarizes the studies on sorption and diffusion of Cs, Sr, Co, Ni, Am and I in common rocks in Finnish bedrock carried out in laboratory experiments. Samples used in these studies were sections of drill cores containing filled and unfilled natural fracture surfaces and drill cores with a diamond drilled longitudinal cavity in the middle of the sample (drill core cups). Samples originated from the two nuclear power plant sites in Finland: tonalite and mica gneiss from Olkiluoto in Eurajoki and rapakivi granite from Haestholmen in Loviisa. The water used in the experiments was synthetic groundwater spiked at a time with one of the radionuclides: Cs-134, Sr-90, Co-60, Ni-63, Am-241 and I-125. Contact times from one week to one year were used to evaluate time dependence of diffusion. An autoradiographic method was used for determination of the penetration depths and diffusion pathways of elements. For determination of diffusion coefficients a quantitative computerized autoradiographic method was used to get the concentration profiles of the radionuclides in the drill cores. Sorption on natural fracture surfaces was more effective than on freshly drilled core samples. Filling materials on natural fracture surfaces, except calcite, increased sorption. The distribution coefficients for drill core cups were about the same as those for unfilled natural fracture surfaces after a contact time of one week and the sorption tendency of radionuclides was: Ka(Cs) > Ka(Co) > Ka(Am) > Ka(Ni) > Ka(Sr) > Ka(I). Radionuclides were observed to penetrate into fissures of the rock matrix and high-capacity minerals. Strontium was found as far as 35 mm in a filled natural fracture surface sample of rapakivi granite after a contact time of one year. The corresponding values were 3.0 mm for cesium, 2.1 mm for cobalt and 2.6 mm for nickel. For americium no diffusion could be observed (a-values for strontium was 6.6 x 10-16-1.1 x 10-13 m2/s, for cesium 4.7 x 10-16-7.2 x 10-15 m2/s

  11. Separation by sequential chromatography of americium, plutonium and neptunium elements: application to the study of trans-uranian elements migration in a European lacustrine system

    International Nuclear Information System (INIS)

    The nuclear tests carried out in the atmosphere in the Sixties, the accidents and in particular that to the power station of Chernobyl in 1986, were at the origin of the dispersion of a significant quantity of transuranic elements and fission products. The study of a lake system, such that of the Blelham Tarn in Great Britain, presented in this memory, can bring interesting answers to the problems of management of the environment. The determination of the radionuclides in sediment cores made it possible not only to establish the history of the depositions and consequently the origin of the radionuclides, but also to evaluate the various transfers which took place according to the parameters of the site and the properties of the elements. The studied transuranic elements are plutonium 238, 239-240, americium 241 and neptunium 237. Alpha emitting radionuclides, their determination requires complex radiochemical separations. A method was worked out to successively separate the three radioelements by using a same chromatographic column. Cesium 137 is the studied fission product, its determination is done by direct Gamma spectrometry. Lead 210, natural radionuclide, whose atmospheric flow can be supposed constant. makes it possible to obtain a chronology of the various events. The detailed vertical study of sediment cores showed that the accumulation mode of the studied elements is the same one and that the methods of dating converge. The cesium, more mobile than transuranic elements in the atmosphere, was detected in the 1963 and 1986 fallout whereas an activity out of transuranic elements appears only for the 1963 fallout. The activity of the 1963 cesium fallout is of the same order of magnitude as that of 1986. The calculation of the diffusion coefficients of the elements in the sediments shows an increased migration of cesium compared to transuranic elements. An inventory on the whole of the lake made it possible to note that the atmospheric fallout constitute the

  12. Design of an Active Photoelectric Isolating RS232/RS485 Converter%一种有源光电隔离RS232/RS485转换器设计

    Institute of Scientific and Technical Information of China (English)

    叶鑫; 李文魁; 高敬东; 钟斌

    2015-01-01

    为了提高转换器的抗干扰能力,根据现场应用环境,设计了一种抗干扰能力较强的有源光电隔离RS232/RS485接口转换电路.介绍了转换器的各电路原理图.测试表明,该转换器结构简单、抗干扰能力强、工作可靠,具有很强的应用价值.

  13. Availability of U-238 and Th-232 present in phosphogypsum used in agriculture: precision and accuracy of the methodology

    Energy Technology Data Exchange (ETDEWEB)

    Malheiro, Luciano H.; Saueia, Catia H.R.; Mazzilli, Barbara P., E-mail: lhmalheiro@ipen.br, E-mail: chsaueia@ipen.br, E-mail: mazzilli@ipen.br [Instituto de Pesquisas Energeticas e Nucleares (IPEN/CNEN-SP), Sao Paulo, SP (Brazil)

    2013-07-01

    Phosphogypsum (PG) can be classified as Technologically Enhanced Naturally Occurring Radioactive Material (TENORM), and it is obtained as a residue of the phosphate fertilizer industry. PG presents in its composition radionuclides of the natural U and Th series: mainly Ra-226, Ra-228, Th-232, Pb-210 and Po-210. The Brazilian producers stock the PG in dry stacks, posing risks to the surrounding environment. A possible solution to this problem is to reuse PG in agriculture; however, it is necessary to ensure that the radionuclides present in the PG will not be available to the agricultural products. This study is part of a research project sponsored by Fundacao de Amparo a Pesquisa do Estado de Sao Paulo (FAPESP - 2010-10587-0) entitled 'Availability of metals and radionuclides in tropical soils amended with phosphogypsum', and its objective is to evaluate the reliability of an optimal methodology to determine U-238 and Th-232 in samples of soils amended with PG through percolation with water. The methodology comprises a sequential radiochemical separation of the radionuclides present in the leachate. The UTEVA resin was used for the purification and separation of U-238 and Th-232, and the final activity concentrations were determined by alpha spectrometry. The precision and accuracy of the methodology were checked by measuring standard reference material. The results obtained for the relative error and relative standard deviation varied respectively from 2.34 % to 5.92 % and 6.10 % to 6.21 % for uranium, and from 0.42 % to 3.13 % and 9.68 % to 10.97 % for thorium. (author)

  14. Influence of DGAT1 K232A polymorphism on milk fat percentage and fatty acid profiles in Romanian holstein cattle.

    Science.gov (United States)

    Tăbăran, A; Balteanu, V A; Gal, E; Pusta, D; Mihaiu, R; Dan, S D; Tăbăran, A F; Mihaiu, M

    2015-01-01

    Milk and dairy products are considered the main sources of saturated fatty acids, which are a valuable source of nutrients in the human diet. Fat composition can be adjusted through guided nutrition of dairy animals but also through selective breeding. Recently, a dinucleotide substitution located in the exon 8 of the gene coding for acyl CoA: diacylglycerol acyltransferase 1 (DGAT1), that alters the amino acid sequence from a lysine to an alanine (p.Lys232Ala) in the mature protein, was shown to have a strong effect on milk fat content in some cattle breeds. Therefore, the objectives of this work were to study the occurrence of the DGAT1 p.Lys232Ala polymorphism in Romanian Holstein cattle and Romanian Buffalo breeds and to further investigate its possible influence on fat percentage and fatty acid profiles. The results obtained in this study show that in Romanian Holstein cattle the K allele is associated with increased fat percentage and higher levels of C16:0 and C18:0 fatty acids. The ratio of saturated fatty acids versus unsaturated fatty acids (SFA/UFA) was also higher in KK homozygous individuals, whereas the fractions of C14:0, unsaturated C18 decreased. The DGAT1 p.Lys232Ala polymorphism revealed a high genetic variance for fat percentage, unsaturated C18, C16:0, and SFA/UFA. Although the effect of this polymorphism was not so evident for short chain fatty acids such as C4:0-C8:0, it was significant for C14:0 fatty acids. We concluded that selective breeding of carriers of the A allele in Romanian Holsteins can contribute to improvement in unsaturated fatty acids content of milk. However, in buffalo, the lack of the A allele makes selection inapplicable because only the K allele, associated with higher saturated fatty acids contents in milk, was identified.

  15. Development of a method for activity measurements of {sup 232}Th daughters with a multidetector gamma-ray coincidence spectrometer

    Energy Technology Data Exchange (ETDEWEB)

    Antovic, N. [Faculty of Natural Sciences and Mathematics, University of Montenegro, Cetinjski put b.b., 81000 Podgorica (Montenegro)], E-mail: antovicn@yahoo.com; Svrkota, N. [Center for Ecotoxicological Research, Put Radomira Ivanovica 2, 81000 Podgorica (Montenegro)

    2009-06-15

    The method for activity measurements of the {sup 232}Th daughters, developed at the six-crystal gamma-ray coincidence spectrometer PRIPYAT-2M and based on coincidence counting of the 583 and 2615 keV photons from cascade transitions which follow {beta}{sup -}-decay of {sup 208}Tl, as well as on counting the 911 keV photons which follow {beta}{sup -}-decay of {sup 228}Ac in the integral and non-coincidence mode of counting, is presented.

  16. 238U, 232TH, AND 222RN concentration measured in various traditional medicinal plant preparation using nuclear track detectors

    International Nuclear Information System (INIS)

    Full text: 238U, 232Th, 222Rn concentrations were measured inside traditional medicinal plants preparations widely used by patients in classic and modern phyto therapy by using a technique based on the use of solid state nuclear track detectors. The intakes of these radionuclides have been determined for adult patients from the ingestion of the studied medical preparations. The influence of mass intake as well as pollution on the contents of the considered radionuclides was investigated. The resulting radiation doses to adult patients from the ingestion of the traditional medical preparations were evaluated.

  17. X-ray variability and prediction of TeV emission in the HBL 1ES1101-232

    OpenAIRE

    Wolter, A.; Tavecchio, F.; Caccianiga, A.; Ghisellini, G.; Tagliaferri, G.

    2000-01-01

    1ES1101-232 is a bright BL Lac of the High frequency peak class. We present here the results of two BeppoSAX observations in which the source has shown a variation of about 30% in flux with a corresponding spectral variability. We interpret the overall spectral energy distribution in terms of an homogeneous SSC model and, by using also the TeV upper limit from a short Mark 6 pointing, derive constraints on the physical parameters of the source, in particular on the magnetic field strength. Th...

  18. An integral experiment on thorium oxide/depleted uranium cylinders with D-T neutrons for 232Th(n, 2n) reaction

    International Nuclear Information System (INIS)

    Highlights: • An integral experiment for 232Th(n, 2n) reaction was carried out on the newly-established ThO2/depleted uranium cylinders. • 232Th(n, 2n) reaction rate distribution was obtained in the assemblies with an uncertainty of about 7%. • Experiments were analyzed by MCNP code with ENDF/B-VI.8, ENDF/B-VII.0, JENDL-4.0 and CENDL-3.1 libraries. • Experimental results could be used to re-evaluate the cross sections of 232Th(n, 2n) reaction. - Abstract: In order to verify the evaluated cross sections of 232Th(n, 2n) reaction for the conceptual design of the thorium based subcritical blanket in the fusion–fission hybrid reactor, an integral experiment on thorium oxide/depleted uranium cylinders was carried out with D-T neutrons using the activation technique. 232Th(n, 2n) reaction rate distribution was obtained at the central axis direction in the assemblies with an uncertainty of about 7%. Experiments were analyzed by using MCNP code with ENDF/B-VI.8, ENDF/B-VII.0, JENDL-4.0 and CENDL-3.1 libraries to validate the nuclear data libraries of 232Th(n, 2n) reaction, the calculated results with JENDL-4.0 agree with the measurements the best with discrepancies within the experimental uncertainty. The average values of C/E for the three benchmark assemblies are 1.058, 1.044 and 0.980. Calculations with different evaluated libraries in the benchmark assemblies show a large discrepancy. The experimental results can be used to re-evaluate the cross sections of the 232Th(n, 2n) reaction

  19. Americium behaviour in plastic vessels

    Energy Technology Data Exchange (ETDEWEB)

    Legarda, F.; Herranz, M. [Departamento de Ingenieria Nuclear y Mecanica de Fluidos, Escuela Tecnica Superior de Ingenieria de Bilbao, Universidad del Pais Vasco (UPV/EHU), Alameda de Urquijo s/n, 48013 Bilbao (Spain); Idoeta, R., E-mail: raquel.idoeta@ehu.e [Departamento de Ingenieria Nuclear y Mecanica de Fluidos, Escuela Tecnica Superior de Ingenieria de Bilbao, Universidad del Pais Vasco (UPV/EHU), Alameda de Urquijo s/n, 48013 Bilbao (Spain); Abelairas, A. [Departamento de Ingenieria Nuclear y Mecanica de Fluidos, Escuela Tecnica Superior de Ingenieria de Bilbao, Universidad del Pais Vasco (UPV/EHU), Alameda de Urquijo s/n, 48013 Bilbao (Spain)

    2010-07-15

    The adsorption of {sup 241}Am dissolved in water in different plastic storage vessels was determined. Three different plastics were investigated with natural and distilled waters and the retention of {sup 241}Am by these plastics was studied. The same was done by varying vessel agitation time, vessel agitation speed, surface/volume ratio of water in the vessels and water pH. Adsorptions were measured to be between 0% and 70%. The adsorption of {sup 241}Am is minimized with no water agitation, with PET or PVC plastics, and by water acidification.

  20. 基于HT46RU232单片机的智能家居电话远程控制系统%A smart home telephone remote control system based on HT46RU232

    Institute of Scientific and Technical Information of China (English)

    谢辉; 王体见; 黄俊森

    2011-01-01

    A smart home telephone remote control system using the telephone communication network,based on HT46RU232 MCU core, matching the MT8870 DTMF decoder chip, ISD2560 voice chip. This system includes user identity verification, remote control home appliances, voice prompts guide the operator, home appliance status query. This system allows the operator to keep abreast of tone under a variety of information about the controlled object, and remote control through telephone number of the controlled object, to achieve intelligent control of the remote appliances.%以HT46RU232单片机为核心,配接DTMF的MT8870解码芯片和ISD2550语音芯片,使用电话通信网络,设计一个智能家居电话远程控制系统.用于校验用户身份、远程控制家用电器、语音提示引导操作、家电状态查询等.可使操作者根据各种提示音及时了解受控对象的有关信息,并通过电话远程控制多个受控对象,实现家电的远程智能化控制.具有推广价值.

  1. Sequential isotopic determination of plutonium, thorium, americium and uranium in the air filter and drinking water samples around the WIPP site

    International Nuclear Information System (INIS)

    The simultaneous determination of actinides in air filter and water samples around the WIPP site have been demonstrated. The analytical method is based on the selective separation and purification by anion exchange and Eichrome-TEVA, TRU and DGA-resin followed by determination of actinides by alpha spectrometry. Counting sources for alpha spectrometric measurements were prepared by microcoprecipitation on neodymium fluoride (NdF3). Radiochemical yields were determined using 242Pu, 229Th, 243Am and 232U as tracers. The validation of the method is performed through the analysis of reference materials or participating in laboratory intercomparison programs. The plutonium concentrations in aerosols varied seasonally, being highest in spring and summer due to the spring-time enhanced wind-storm transportation of radioactive aerosols from the stratosphere to the troposphere. The 238Pu/239+240Pu activity ratio in the aerosol samples is typically close to that of global fallout from historic above-ground nuclear weapons testing. The results presented here indicate that the source of plutonium in the WIPP environment results mainly from global nuclear fallout and there is no evidence of increases in radiological contaminants in the region that could be attributed to releases from the WIPP. (author)

  2. Determination of specific concentrations of {sup 40}K, {sup 238}U and {sup 232}Th in mineral fertilizer samples

    Energy Technology Data Exchange (ETDEWEB)

    Garcez, Ricardo W.D.; Lopes, Jose M.; Silva, Ademir X., E-mail: r.w.o.g@fisica.if.uff.br, E-mail: ademir@nuclear.ufrj.br [Coordenacao dos Programas de Pos-Graduacao em Engenharia (COPPE/UFRJ), Rio de Janeiro, RJ (Brazil). Programa de Engenharia Nuclear; Domingues, Alessandro M.; Lima, Marco F. [Universidade Federal Fluminense (UFF), Niteroi, RJ (Brazil)

    2015-07-01

    The use of fertilizer is an established practice worldwide to promote agricultural productivity increased without increasing the planted area, resulting in native forests protection and increase of the food availability. Some kinds of fertilizer have in their chemical composition some radionuclides due the origin of its feedstock, such as {sup 238}U, the {sup 232}Th, and their descendants, beyond {sup 40}K. Knowledge of the radioactivity levels in the environment is great importance to know the gamma radiation dose that the human being is exposed. For identification and quantitation of radionuclides, it was used gamma spectrometry where HPGe detector was used to obtain the spectra, and LabSOCS software for calculating the detection efficiency for each energy. The values of {sup 232}Th specific concentrations ranged from 4.1 to 368.1 Bq.Kg{sup -1}, the values of {sup 238}U specific concentrations ranged from 16.0 to 647.7 Bq.Kg{sup -1} and {sup 40}K specific concentrations ranged from 19.1 to 12713 Bq.Kg{sup -1}. Concentrations of values are consistent with those found in literature. (author)

  3. Primordial radioactivity ((238)U, (232)Th and (40)K) measurements for soils of Ludhiana district of Punjab, India.

    Science.gov (United States)

    Badhan, K; Mehra, R

    2012-11-01

    The aim of the present work was to study the activity concentration and absorbed gamma dose rates due to primordial radionuclides ((238)U, (232)Th and (40)K) for the soil of different villages of Ludhiana district of Punjab, India using a high-purity germanium detector based on high resolution gamma-ray spectrometry. The average activity concentrations of (238)U, (232)Th and (40)K in the soil samples have been found to be 28.58, 50.95 and 569.59 Bq kg(-1), respectively, which gives the total gamma dose rate contribution of 68.50 nGy h(-1). To evaluate the radiological hazard of the natural radioactivity, the radium equivalent activity, the external hazard index, the absorbed dose rate and the effective dose rate have been calculated. The calculated radium equivalent activity values are on the lower side of the recommended safe limit value of 370 Bq kg(-1) by Organization of Economic and Control Department. The calculated value of external health hazard index is lower than unity. PMID:22899219

  4. Investigation of resonance structure and Doppler-effect of cross sections for 232 Th, 235 U and 239 Pu

    International Nuclear Information System (INIS)

    The results of measuring the neutron transmissions for 232 Th, 235 U and 239 Pu metal samples carried out at the 60 m, 123 m and 1006 m flight paths of the Dubna IBR-30 booster in the neutron energy range of 2 eV - 200 keV are given and discussed. The measurements were made at the room and liquid nitrogen temperatures. The batteries of 3 boron and 26 helium counters were used as detectors. The results of the calculations of analogous transmissions realized on the base of the evaluated data libraries BROND-2, ENDF/B-6 and JENDL-3 by means of the GRUCON computer program package are also given. It is concluded that the 235 U Doppler coefficients and effective total cross sections taken from measured transmissions are in a good agreement with calculation results based on the ENDF/B-6 library at energies of 2.15 eV - 200 keV. The BROND-2 and JENDL-3 parameters give the Doppler coefficients and effective cross sections which are 10-30% higher than the experimental and ENDF/B-6 ones at the resonance energies of 46.5 - 465 eV. For 239 Pu there is agreement of the experimental and calculational results within the experimental error limits. For 232 Th experimental values for the Doppler coefficients and effective cross sections are 10-15% higher than the calculated ones with all libraries in resonance energy region. 9 refs., 2 tabs., 1 fig

  5. Deactivation and cleanout of the 308 Fuels Laboratory and the 232-Z Incinerator at the Hanford site

    International Nuclear Information System (INIS)

    This paper describes the deactivation and source term reduction activities conducted over the recent past in two plutonium-contaminated Hanford Site buildings: the 308 Fuels Development Laboratory and the 232-Z Incinerator. Both of these facilities belong to the U.S. Department of Energy, and the projects are unique success stories carried out in direct support of EM-60 functions and requirements. In both cases the buildings, for different reasons, contained unacceptable amounts of plutonium, and were stabilized and placed in a safe, pre-D ampersand D (decontamination and decommissioning) mode. The concept of deactivation as the last step in the operating life of a facility will be discussed. The need for and requirements of EM-60 transition between operations and D ampersand D, the costs savings, techniques, regulations and lessons learned also will be discussed. This paper describes the strategies that led to successful source term reduction: accurate characterization, cooperation among different divisions within DOE and the Hanford Site, attention to regulations (especially unique in this case since the 232-Z Incinerator has been nominated as a Historic Structure to the National Register of Historic Places), and stakeholder concerns involving the proximity of the 308 Building to the Columbia River. The paper also weaves in the history, missions, and plutonium accumulation of the two buildings. The lessons learned are cogent to many other present and future deactivation activities across the DOE complex and indeed across the world

  6. [Trends in infective endocarditis in a medium-sized University Hospital in Italy: analysis of 232 cases].

    Science.gov (United States)

    Pallotto, Carlo; Martinelli, Laura; Baldelli, Franco; Bucaneve, Gianpaolo; Cecchini, Enisia; Malincarne, Lisa; Pasticci, Maria Bruna

    2014-06-01

    The aim of this study was to evaluate the epidemiological and clinical characteristics of 232 cases of infective endocarditis (IE), admitted to the Clinica delle Malattie Infettive of Perugia Italy from 1973 to 2012. The analysis was retrospective until 2004. After this year, all the consecutive IE cases were included by utilizing the same prospective observational protocol of the Italian Study on Endocarditis (SEI). Out of 232 EI cases, 200 (86.2 %) were definite. Over the 40-year period, a statistically significant increase was observed in the patients' age, the rate of IE admissions and prosthetic device IEs. The rate of healthcare-associated IEs also increased in the last 10 years (p=NS). Diabetes mellitus was the most frequent comorbidity. There were no variations in the rate of S. aureus and streptococcal IEs. Central nervous system complications and surgery were reported in 19.4 percent and 29.3 percent of the cases, respectively. The in-hospital mortality was 18.9 percent. In conclusion, the epidemiological and clinical trends of this study are in agreement with the literature. The difference in S. aureus endocarditis, neurological complications and surgery rates may be due to the fact that this was a single centre and, for its first part, a retrospective study. A shared, multidisciplinary protocol may be useful to improve the outcome of patients with IE and its epidemiology.

  7. EURADOS action for determination of americium in skull measures in vivo and Monte Carlo simulation; Accion EURADOS para la determinacion de americio en craneo mediante medidas in-vivo y simulacion Monte Carlo

    Energy Technology Data Exchange (ETDEWEB)

    Lopez Ponte, M. A.; Navarro Amaro, J. F.; Perez Lopez, B.; Navarro Bravo, T.; Nogueira, P.; Vrba, T.

    2013-07-01

    From the Group of WG7 internal dosimetry of the EURADOS Organization (European Radiation Dosimetry group, e.V.) which It coordinates CIEMAT, international action for the vivo measurement of americium has been conducted in three mannequins type skull with detectors of Germanium by gamma spectrometry and simulation by Monte Carlo methods. Such action has been raised as two separate exercises, with the participation of institutions in Europe, America and Asia. Other actions similar precede this vivo intercomparison of measurement and modeling Monte Carlo1. The preliminary results and associated findings are presented in this work. The laboratory of the body radioactivity (CRC) of service counter of dosimetry staff internal (DPI) of the CIEMAT, it has been one of the participants in vivo measures exercise. On the other hand part, the Group of numerical dosimetry of CIEMAT is participant of the Monte Carlo2 simulation exercise. (Author)

  8. Critical and shielding parametric studies with the Monte Carlo code TRIPOLI to identify the key points to take into account during the transportation of blanket assemblies with high ratio of americium

    International Nuclear Information System (INIS)

    In the framework of French research program on Generation IV sodium cooled fast reactor, one possible option consists in burning minor actinides in this kind of Advanced Sodium Technological Reactor. Two types of transmutation mode are studied in the world : the homogeneous mode of transmutation where actinides are scattered with very low enrichment ratio in fissile assemblies and the heterogeneous mode where fissile core is surrounded by blanket assemblies filled with minor actinides with ratio of incorporated actinides up to 20%. Depending on which element is considered to be burnt and on its content, these minor actinides contents imply constraints on assemblies' transportation between Nuclear Power Plants and fuel cycle facilities. In this study, we present some academic studies in order to identify some key constraints linked to the residual power and neutron/gamma load of such kind of blanket assemblies. To simplify the approach, we considered a modeling of a 'model cask' dedicated to the transportation of a unique irradiated blanket assembly loaded with 20% of Americium and basically inspired from an existent cask designed initially for the damaged fissile Superphenix assembly transport. Thermal calculations performed with EDF-SYRTHES code have shown that due to thermal limitations on cladding temperature, the decay time to be considered before transportation is 20 years. This study is based on explicit 3D representations of the cask and the contained blanket assembly with the Monte Carlo code TRIPOLI/JEFF3.1.1 library and concludes that after such a decay time, the transportation of a unique Americium radial blanket is feasible only if the design of our model cask is modified in order to comply with the dose limitation criterion. (author)

  9. MBE-grown 232-270 nm Deep-UV LEDs using Monolayer thin Binary GaN/AlN quantum heterostructures

    CERN Document Server

    Islam, SM; Verma, Jai; Protasenko, Vladimir; Rouvimov, Sergei; Xing, Huili; Jena, Debdeep

    2016-01-01

    Electrically injected deep ultra-violet (UV) emission is obtained using monolayer (ML) thin GaN/AlN quantum structures as active regions. The emission wavelength is tuned by controlling the thickness of ultrathin GaN layers with monolayer precision using plasma assisted molecular beam epitaxy (PAMBE). Single peaked emission spectra is achieved with narrow full width at half maximum (FWHM) for three different light emitting diodes (LEDs) operating at 232 nm, 246 nm and 270 nm. 232 nm (5.34 eV) is the shortest EL emission wavelength reported so far using GaN as the light emitting material and employing polarization-induced doping.

  10. Radioactivity of 238U, 232Th, 40K, and 137Cs and assessment of depleted uranium in soil of the Musandam Peninsula, Sultanate of Oman

    OpenAIRE

    SALEH, Ibrahim Hindawy

    2012-01-01

    238U, 232Th, 40K, and 137Cs radioactivities were determined in soil samples collected from the Musandam Peninsula, Sultanate of Oman, using a high resolution gamma-ray spectroscopy system. In addition, total uranium was measured in selected soil samples by inductively coupled plasma optical emission spectroscopy (ICP-OES). The averages of radioactivity levels in the soil for 238U, 232Th, and 40K were 14.42 Bq kg-1, 9.95 Bq kg-1, 158.21 Bq kg-1, and 2770 Bq m-2 for 137Cs, respectively...

  11. 232例儿童热性惊厥血清钠浓度临床分析%Clinical Analysis about Concentrations of Natrium in 232 Cases Children with Febrile Convulsions

    Institute of Scientific and Technical Information of China (English)

    刘庆玲

    2013-01-01

    Objective:To investigate the changes of concentrations of natrium and its clinical significance in children with febrile convulsions. Method:Clinical data of 232 children with febrile convulsions who visited Beijing commercial aviation general hospital from 2010 to 2012 were retrospectively analyzed.Result:The concentrations of natrium of children with febrile convulsions were diffrently lower than normal,especially in children with recurrent convulsion and status convulsion whose concentrations of natrium were obviously lower than children with simple febrile convulsions. Conclusion:Varying degrees of hyponatremia occur in children with febrile convulsions. It should pay attention to correct hyponatremia in treatmen of febrile convulsions to reduce the relapse frequency and duration of febrile convulsions,so reduce the harm of brain organization.%目的:探讨热性惊厥患儿血清钠浓度变化及临床意义。方法:对北京民航总医院2010-2012年急诊治疗的232例热性惊厥患儿血清钠浓度作回顾性分析。结果:热性惊厥儿童血清钠浓度常有不同程度的降低,且惊厥反复发作及惊厥持续状态患儿的血清钠浓度明显低于单纯性热性惊厥患儿。结论:热性惊厥患儿常存在不同程度的低钠血症,在常规治疗小儿热性惊厥时应注意纠正低钠血症,以减少小儿热性惊厥的发作次数及持续时间,减轻脑组织损害。

  12. Measurement of neutron-transmission spectra through 232Th from 8 MeV to 4 keV

    International Nuclear Information System (INIS)

    Neutron transmission spectra through room-temperature 232Th samples have been measured by use of the time-of-flight technique, the ORELA pulsed neutron source, and a 1-mm-thick Li-glass detector. The measurement and data reduction are described in detail. The 40-m transmission spectra through eight samples are directly compared from 15 to 4000 eV with resolution-broadened transmission spectra calculated from the ENDF/B-V total cross section. Two sets of 22-m transmission spectra through five samples are combined into one total cross section from 0.008 to 15.0 eV and compared with the ENDF/B-V evaluation. 13 figures, 12 tables

  13. Proposal and application of methodology for monitoring workers occupationally exposed to Thorium-232 and its decay products

    International Nuclear Information System (INIS)

    Thorium-232 is the parent of one of the naturally occurring decay series and is widely spread on the earth's crust, being also present in higher concentrations at some deposits located mainly in Brazil and India. The occupational exposure to this radionuclide may occur in several steps of the thorium cycle. In Brazil, there is a large number of workers that should be monitored because they manipulate directly or indirectly different kinds of ores, raw materials and products containing significant amounts of thorium in its composition. In this study, the techniques developed specifically for the in vivo and in vitro monitoring of these workers are presented together with the application of these techniques to a group of selected workers classified as occupationally exposed. It is also presented the methodology by which the results obtained with these measurements are interpreted with the objective of identifying the main pathways of incorporation and reducing the internal doses to values as low as reasonably achievable. (author)

  14. 基于FS8610的RS232-Ethernet应用的设计与实现

    Institute of Scientific and Technical Information of China (English)

    沙健胜; 刘晓升

    2008-01-01

    主要介绍了基于FS8610芯片而实现串口服务器功能的设计方案,采用一个集成了网络协议功能的8位高速控制芯片,通过C编程实现串口与以太网之间的数据通信。串口至以太网接口转换器使得带有RS232/422/485通讯接口的设备和以太网服务器进行数据流传输,通过以太网服务器对串口设备进行实时监控。

  15. Challenges and solutions for random sampling of parameters with extremely large uncertainties and analysis of the 232Th resonance covariances

    International Nuclear Information System (INIS)

    Covariance data in the existing evaluated nuclear data libraries often include large relative uncertainties and mathematical inconsistencies, which arise especially in combination with random sampling. The 232Th evaluation from the ENDF/B-VII.1 library has been taken as an example. Possible solutions for mathematically impossible correlation matrices with negative eigenvalues and too low correlation coefficients between inherently positive parameters with large relative uncertainties are proposed. Convergence of the random sampling for lognormal distribution with extremely high relative standard deviations is slow by nature. Using weighted sampling, single parameters or a limited number of correlated parameters with large uncertainties can be sampled. Efficient sampling of a large number of correlated parameters with extremely large relative uncertainties remains unsolved

  16. Detection efficiencies of 226Ra and 232Th in different modes of counting of the PRIPYAT-2M spectrometer

    Directory of Open Access Journals (Sweden)

    Antović Nevenka M.

    2009-01-01

    Full Text Available Detection efficiencies of 226Ra and 232Th decay products, as well as corresponding minimum detectable activities in different modes of counting of the PRIPYAT-2M spectrometer (integral, when all pulses - coincident and non-coincident, are counted; non-coincident, when only non-coincident pulses are counted; coincident, when coincident pulses of multiplicity from 2 to 6 are counted, in energy ranges of 200 keV to 2000 keV and 300 keV to 3000 keV are presented here. It has been shown that the mode of double coincidences is the optimum one for measuring radium and thorium activity. In this mode of counting, the sensitivity of the spectrometer is the highest.

  17. Subcontracting strategy for the decontamination and decommissioning of Savannah River Site's First Tritium Extraction Facility, 232-F

    International Nuclear Information System (INIS)

    The Savannah River Site (SRS) has been actively proceeding with the decontamination and decommissioning (D and D) of various facilities and structures which were instrumental in the success of past missions at the site. The most ambitious of these efforts involves the subcontracting of the complete D and D of the first SRS Tritium Extraction Facility, identified as building 232-F. This facility operated in the mid 1950's and discontinued operations permanently in 1958. The approach utilized for this effort attempts to invoke the novel principle of open-quotes As Commercial As Reasonably Achievableclose quotes or open-quotes ACARAclose quotes. This concept of ACARA applies only the minimum essential requirements necessary to successfully perform the D and D task. Integral to this approach is the subcontractor provision for maximum flexibility in the identification of and adherence to the requirements of applicable DOE Orders, federal, state and local laws and regulations, as well as site specific procedures without violating the site contractual requirements. The technical specification prepared for this effort provides the basis for a competitively bid contract to perform the entire D and D evolution, including initial facility characterization, waste stream characterization and certification, D and D and waste disposal. Preparation and development of this specification and the subsequent Request For Proposal (RFP) was a successful team oriented endeavor. The schedule for this fast-track undertaking took three months to complete. Successful initiation of this task will be the first D and D of a facility containing both radioactive and hazardous material at an operating site within the DOE Weapons Complex. The strategy for preparing the D and D subcontract for the 232-F structure was facilitated by applying the ACARA principle. This approach resulted in the accelerated development of the specification and RFP documents, as well as minimized the complexities of

  18. Avian influenza (H5N1 virus of clade 2.3.2 in domestic poultry in India.

    Directory of Open Access Journals (Sweden)

    Shanmuga Nagarajan

    Full Text Available South Asia has experienced regular outbreaks of H5N1 avian influenza virus since its first detection in India and Pakistan in February, 2006. Till 2009, the outbreaks in this region were due to clade 2.2 H5N1 virus. In 2010, Nepal reported the first outbreak of clade 2.3.2 virus in South Asia. In February 2011, two outbreaks of H5N1 virus were reported in the State of Tripura in India. The antigenic and genetic analyses of seven H5N1 viruses isolated during these outbreaks were carried out. Antigenic analysis confirmed 64 to 256-fold reduction in cross reactivity compared with clade 2.2 viruses. The intravenous pathogenicity index of the isolates ranged from 2.80-2.95 indicating high pathogenicity to chickens. Sequencing of all the eight gene-segments of seven H5N1 viruses isolated in these outbreaks was carried out. The predicted amino acid sequence analysis revealed high pathogenicity to chickens and susceptibility to the antivirals, amantadine and oseltamivir. Phylogenetic analyses indicated that these viruses belong to clade 2.3.2.1 and were distinct to the clade 2.3.2.1 viruses isolated in Nepal. Identification of new clade 2.3.2 H5N1 viruses in South Asia is reminiscent of the introduction of clade 2.2 viruses in this region in 2006/7. It is now important to monitor whether the clade 2.3.2.1 is replacing clade 2.2 in this region or co-circulating with it. Continued co-circulation of various subclades of the H5N1 virus which are more adapted to land based poultry in a highly populated region such as South Asia increases the risk of evolution of pandemic H5N1 strains.

  19. Effects of the diacylglycerol o-acyltransferase 1 (DGAT1) K232A polymorphism on fatty acid, protein, and mineral composition of dairy cattle milk

    NARCIS (Netherlands)

    Bovenhuis, H.; Visker, M.H.P.W.; Poulsen, N.A.; Sehested, J.; Valenberg, van H.J.F.; Arendonk, van J.A.M.; Larsen, L.B.; Buitenhuis, A.J.

    2015-01-01

    Several studies have described associations between the diacylglycerol o-acyltransferase 1 (DGAT1) K232A polymorphism and routinely collected milk production traits but not much is known about effects of the DGAT1 polymorphism on detailed milk composition. The aim of this study was to estimate ef

  20. Prototype of A/Duck/Sukoharjo/Bbvw-1428-9/2012 subtipe H5N1 clade 2.3.2 as vaccine on local duck

    Directory of Open Access Journals (Sweden)

    Risa Indriani

    2014-06-01

    Full Text Available A/Duck/Sukoharjo/Bbvw-1428-9/2012 virus subtipe H5N1 clade 2.3.2 as seed vaccine on local duck. AI H5N1 clade 2.3.2 vaccine containing 256 HAU per dose was formulated using adjuvant ISA 71VG Montanide ™. Six groups of one day old local duck were used in this study. Three groups (10 ducks per group were vaccinated and 3 groups (9 duck per group were served control. Vaccination was conducted when the duck were three weeks old of age using single dose. Three weeks after vaccination when the duck were challenged either with HPAI H5N1 clade 2.3.2, or HPAI H5N1 clade 2.1.3 virus at dose 106 EID50/ 0.1 ml by drops intranasaly. Result showed that vaccination produced 100% protection compared to unvaccinated ducks againt HPAI subtipe H5N1 clade 2.3.2, and 100% protection againt HPAI H5N1 clade 2.1.3 (A/ck/wj/Subang-29/2007 and A/ck/wj/Smi-Part/2006, while unvaccinated ducks showed virus shedding on day 3 post infection.

  1. Distribution of 226Ra, 232Th and 40K in soils and sugar cane crops at Corumbatai river basin, Sao Paulo State, Brazil

    International Nuclear Information System (INIS)

    The common use of phosphate fertilizers NPK and amendments in sugar cane crops in Brazilian agriculture may increase the 226Ra, 232Th and 40K activity concentrations in soils and their availability for plants and human food chain. Thus, the main aim of this study was to evaluate the distribution of 226Ra, 232Th and 40K in soils and sugar cane crops in the Corumbatai river basin, Sao Paulo State, Brazil. The gamma spectrometry was utilized to measure the 226Ra, 232Th and 40K activity concentration in all samples. The soil-to-sugar cane transfer factors (TF) were quantified using the ratio between the radionuclide activity concentration in sugar cane and its activity concentration in soil. The results show that, although radionuclides incorporated in phosphate fertilizers and amendments are annually added in the sugar cane crops, if utilized in accordance with the recommended rates, their use does not lead to hazards levels in soils. The soil-to-sugar cane transfer of radionuclides occurred in the following order 40K>226Ra>232Th. Therefore, under these conditions, radionuclides intake through consumption of sugar is not hazardous to human health.

  2. Proton-induced fission at 190 MeV of W-nat, Au-197, Pb-nat, Pb-208, and Th-232

    NARCIS (Netherlands)

    Duijvestijn, MC; Koning, AJ; Beijers, JPM; Gastal, M; van Klinken, J; Ostendorf, RW

    1999-01-01

    Proton-induced fission at 190 MeV of W-nat, Au-197, Pb-nat, Pb-208, and Th-232 is studied by means of an innovative method based on activation analysis. The fission-product mass distribution is reconstructed from the fission-product yields, which are obtained from off-line observed gamma-ray spectra

  3. Comment on `Update of 40K and 226Ra and 232Th series $\\gamma$-to-dose conversion factors for soil'

    CERN Document Server

    Malins, Alex; Saito, Kimiaki

    2015-01-01

    A letter to the editor of the Journal of Environmental Radioactivity on the article: E. Gasser, A. Nachab, A. Nourreddine, Ch. Roy, and A. Sellam, `Update of 40K and 226Ra and 232Th series $\\gamma$-to-dose conversion factors for soil', J. Environ. Radioactiv. 138, 68-71 (2014), DOI: 10.1016/j.jenvrad.2014.08.002.

  4. Measurement of Fragment Mass Distributions in Neutron-induced Fission of {sup 238}U and {sup 232}Th at Intermediate Energies

    Energy Technology Data Exchange (ETDEWEB)

    Simutkin, V.D. [Uppsala University, P.O Box 525, SE-751 20 Uppsala (Sweden)

    2008-07-01

    Conceptual analysis of accelerator-driven systems assumes extensive use of nuclear data on neutron-induced reactions at intermediate energies. In particular, information about the fission fragment yields from the {sup 238}U(n,f) and {sup 232}Th(n,f) reactions is of particular interest at neutron energies from 10 to 200 MeV. However, there is a lack of such data for both {sup 238}U and {sup 232}Th. Up to now, the intermediate energy measurements have been performed for {sup 238}U only, and there are no data for the {sup 232}Th(n,f) reaction. The aim of the work is to provide such data. Fission fragment mass distributions for the {sup 232}Th(n,f) and {sup 238}U(n,f) reactions have been measured for the incident neutron energies 32.8 MeV, 45.3 MeV and 59.9 MeV. The experiments have been performed at the neutron beam facility of the Universite Catholique de Louvain, Belgium. A multi-section Frisch-gridded ionization chamber has been used as a fission fragment detector. The data obtained have been interpreted in terms of the multimodal random neck-rupture model (MMRNRM). (authors)

  5. The activity concentrations of 40K, 226Ra, 232Th, 238U and 7Be in moss from spas in eastern Serbia in the period 2000-2012

    Directory of Open Access Journals (Sweden)

    Čučulović Ana

    2014-01-01

    Full Text Available In this work we present the activity concentrations of natural radionuclides 40K, 226Ra, 232Th, 238U and 7Be in mosses. One hundred and sixty-seven moss samples were collected between 2001 and 2012 from the territory of the Sokobanja, Banja Jošanica and Gamzigradska Banja spas. They were classified into 23 species. The activity concentrations (Bq/kg in moss from Sokobanja spa were: 40K 25-427; 226Ra 0.3-36; 232Th 1.0-37; 238U 0.4-28 and 7Be 29-210; from Banja Jošanica spa they were: 40K 90-242; 226Ra 2.4-11.7; 232Th 2.0-12.7; 238U 1.6-11.3 and 7Be 142-212; Gamzigradska Banja spa: 40K 95-351; 226Ra 8.0-21; 232Th 5.1-19; 238U 6.7-18 and 7Be 20-144. The activity concentrations of dominant natural radionuclides (potassium, radium, thorium and uranium in the moss samples were within the usual ranges for the territory of Serbia. [Projekat Ministarstva nauke Republike Srbije, br. III 43009

  6. [A case of Creutzfeldt-Jakob disease with a double mutation (V180I/M232R) in the PRNP gene].

    Science.gov (United States)

    Koh, Kishin; Takaki, Ryusuke; Miwa, Michiaki; Nagasaka, Takamura; Shindo, Kazumasa; Takiyama, Yoshihisa

    2015-01-01

    Creutzfeldt-Jakob disease (CJD) presents with rapidly progressive dementia associated with several symptoms including pyramidal, extrapyramidal, and cerebellar signs. In Japan, patients with PRNP gene mutations comprise 18.3% of CJD cases. In the present study, we report a 74-year-old man with a double mutation in the PRNP gene. He showed dysarthria, gait disturbance, and cognitive impairment. High signal intensity was observed in the bilateral cortex on brain MRI in diffusion-weighted images. There were high total Tau protein and 14-3-3 protein levels in the cerebrospinal fluid. We diagnosed him as having CJD clinically, and analyzed the PRNP gene, which revealed a V180I mutation and a M232R one, i.e., a compound heterozygous status. In our patient, the disease has very slowly progressive (total disease course, 37 months). The V180I and M232R mutations are specific mutations to Japanese CJD patients. For patients with a double PRNP gene mutation, only V180I and M232R have been known. Patients with a double mutation (V180I /M232R) in the PRNP gene might show an atypical disease course with a slow progression. PMID:26103817

  7. ESPON 2.3.2: GOVERNANCE OF TERRITORIAL AND URBAN POLICIES FROM EU TO LOCAL LEVEL (2004-2006) : National Overview: France

    OpenAIRE

    Santamaria, Frédéric; Bonerandi, Emmanuelle

    2005-01-01

    Rapport d'étude fourni au pilote du projet (université de Valence, Espagne) dans le cadre du programme ESPON National overview for France dealing with territorial and urban governance realised in the framework of the ESPON project 2.3.2

  8. Statistical model calculations of pre-scission neutron multiplicity for the heavy ion induced fusion-fission reactions with actinide target 232Th

    Directory of Open Access Journals (Sweden)

    Thakur Meenu

    2015-01-01

    Full Text Available The reaction mechanism of 19F + 232Th and 28Si + 232Th systems populating the near-super-heavy compound nuclei 251Es and 260Rf respectively are investigated using neutron multiplicity as a probe. The prescission neutron multiplicities of these compound nuclei are calculated at different excitation energies using a statistical model code. These calculations are performed using the Bohr-Wheeler transition state fission width as well as the dissipative dynamical fission width based on the Kramers’ prescription. For 19F + 232Th system, the measured yield of pre-scission is compared with the statistical model calculations for the decay of a compound nucleus in the excitation energy range of 54-90 MeV. The comparison between the measured and the calculated values indicates that the Bohr-Wheeler fission width underestimates the pre-scission neutron yield and a large amount of dissipation strength is required to reproduce the experimental pre-scission neutron multiplicities. The excitation energy dependence of the fitted values of the dissipation coefficient is also discussed. In addition, exploratory statistical model calculations of pre-scission neutron multiplicity for the 28Si + 232Th system are presented in the above range of excitation energy.

  9. Speciation analysis of 129I, 137Cs, 232Th, 238U, 239Pu and 240Pu in environmental soil and sediment

    DEFF Research Database (Denmark)

    Qiao, Jixin; Hansen, Violeta; Hou, Xiaolin;

    2012-01-01

    The environmental mobility and bioavailability of radionuclides are related to their physicochemical forms, namely species. We here present a speciation analysis of important radionuclides including 129I (also 127I), 137Cs, 232Th, 238U and plutonium isotopes (239Pu and 240Pu) in soil (IAEA-375...

  10. Intake of 238U and 232Th through the consumption of foodstuffs by tribal populations practicing slash and burn agriculture in an extremely high rainfall area

    International Nuclear Information System (INIS)

    The concentration of naturally occurring radionuclides 232Th, 238U was determined using Instrumental Neutron Activation Analysis (INAA) in different food groups namely cereals, vegetables, leafy vegetables, roots and tubers cultivated and consumed by tribal population residing around the proposed uranium mine. The study area is a part of rural area K. P. Mawthabah (Domiasiat) in the west Khasi Hills District of Meghalaya, India located in the tropical region of high rainfall that remains steeped in tribal tradition without much outside influence. Agriculture by Jhum (slash and burn) cultivation and animal husbandry are the main occupation of the tribal populations. A total of 89 samples from locally grown food products were analyzed. The concentration of 238U and 232Th in the soil of the study area was found to vary 1.6–15.5 and 2.0–5.0 times respectively to the average mean value observed in India. The estimated daily dietary intake of 238U and 232Th were 2.0 μg d−1 (25 mBq d−1) and 3.4 μg d−1 (14 mBq d−1) is comparable with reported range 0.5–5.0 μg d−1 and 0.15–3.5 μg d−1 respectively for the Asian population. - Highlights: ► 232Th, 238U were determined using Instrumental Neutron Activation Analysis (INAA). ► Study area located in the tropical region of high rainfall that remains steeped in tribal tradition. ► Agriculture by Jhum (slash and burn) cultivation and animal husbandry are the main occupation of the tribal populations. ► The estimated daily intake of 232Th and 238U in high rainfall area was found to be 3.4 and 2.0 μg respectively.

  11. 宫颈不典型鳞状细胞232例临床分流方法探讨%Clinical Sorting Method of 232 Cases with Atypical Squamous Cells

    Institute of Scientific and Technical Information of China (English)

    杨冬; 诸雪峻

    2011-01-01

    Objective:To explore the correct diagnosis and proper sorting method in women with ASC. Methods:232 Women diagnosed as ASC were included in this study, and underwent colposcopy and hr-HPV test (Hybrid Capture 2). Results:(I)ln the 232 cases of ASC, 214 cases of ASCUS ( 92.2%)and 18 cases of ASCH (7. 8%) were found. ?The positive result of cervical biopsy and CIN11 or higher grade lesion in ASCUS or ASCH groups were 98 cases(45. 8%) ,18 caes(8.4%) ,and 15 cases(83.3%), 6 cases (33. 3%) ,the differences between the two groups were significant (P=0. 003;P=0. 005). In cases with ASCUS, 97 cases of hr-HPV Test were positive, in which 77.3% cases were with positive biopsy, 16. 5% cases were CIN U or higher grade disease. While, 117 cases of HPV test were negative, in which 19.7% cases were positive biopsy, 1.7% cases were CIN n , no higher grade disease. (3)The sensitivity and specificity of hr-HPV test for CIN and cervical cancer were 76. 5% and 81.0%, while those of colposcopy were 83.7% and 77.6% respectively, no differences were found between the two groups( P=0.283; P=0.627). Conclusions: ASCH strongly predicts the presence of HSIL and cervical cancer, colposcopic examination is the proper choice. HPV test and colposcopic examination are effective sorting methods for patients with ASCUS. For HPV negative patients, repeat pap smear in 6 month is proper, while for HPV positive patients,colposcopic examination is recommended.%目的:探讨宫颈不典型鳞状细胞(ASC)正确诊断、合理临床分流方法.方法:232例ASC患者接受阴道镜下宫颈活检,并采用第二代杂交捕获法检测高危型人乳头瘤病毒(HPV).结果:①232例ASC中未明确诊断意义的不典型鳞状上皮细胞(ASCUS)Z14例(92.2%),不排除高度病变的不典型鳞状上皮细胞(ASCH)18例(7.8%).②ASCUS组和ASCH组宫颈活检阳性患者、CINⅡ-Ⅲ及宫颈浸润癌患者分别为98例(45.8%)、18例(8.4%)和15例(83.3%)、6例(33.3%),两组间比较差

  12. Analysis of chromosomal karyotypes, age and height on diagnosis of 232 patients with Turner syndrome%Turner综合征232例染色体核型、诊断年龄和身高分析

    Institute of Scientific and Technical Information of China (English)

    王红; 金煜炜; 瞿宇晋; 宋昉

    2013-01-01

    目的 研究Turner综合征(TS)的染色体核型、诊断年龄和身高的分布特点.方法 对27年随机就诊的1015例身材矮小女童,经过染色体核型分析确定TS的诊断,回顾性统计分析TS患儿的染色体核型、诊断年龄和身高,采用SPSS 11.0软件进行数据统计分析.结果 1.确诊TS患儿232例,诊断率为22.9%.2.共检测到26种异常染色体核型,以45,X和46,Xi(Xq)最为常见,分别为75例(32.4%)和38例(16.4%).其中有21种嵌合体核型,共111例(47.8%).3.TS患儿诊断年龄为(10.90 ±4.55)岁,青春期是诊断高峰.<2岁组15例(6.4%)、2~<7岁组35例(15.1%)、7~ <12岁组93例(40.1%)、12 ~<18岁组89例(38.4%).4.TS患儿身高标准差得分(Z分值)均值为-3.60±1.20,Z分值与诊断年龄之间存在明显的负线性相关(r=-0.613,P<0.000).5.在年龄≥13岁的74例TS患儿中64例(86.5%)出现青春期延迟,而在81例非TS病例中仅22例(27.2%),2组间差异有统计学意义(OR=16.297,P=0.000).结论 1.TS的染色体核型呈多样性.2.TS患儿的身高不足随着年龄的增加更为显著,青春期延迟的特征性表现也逐渐显现.3.国内TS诊断年龄比发达国家延迟;对于身高Z分值低于-2或在身高下限的矮小女童应及早进行染色体核型分析,有益于TS的早期诊断.%Objective To study the distribution characteristics of chromosomal karyotypes,age and height on diagnosis of patients with Turner syndrome(TS).Methods Karyotypes analysis was performed in 1015 girls with short stature who visited the hospital in recent 27 years.And statistical analysis of the chromosomal karyotypes,age and height on the diagnosis of patients with TS were performed by using the SPSS 11.0 software.Results 1.Two hundred and thirty-two (22.9%) patients were diagnosed with TS.2.A total of 26 kinds of abnormal karyotypes were detected in 232 patients with TS and the 45,X (32.4%,75/232 cases) and 46,Xi (Xq) (16.4%,38/232 cases) were

  13. Measurement of the {sup 232}thorium capture cross section at n-TOF-CERN; Mesure de la section efficace de capture neutronique du {sup 232}Th a n-TOF au CERN

    Energy Technology Data Exchange (ETDEWEB)

    Aerts, G

    2005-09-01

    Within the context of nuclear power as a sustainable energy resource, a program of research is concentrated on a new nuclear fuel cycle based on thorium. The main advantage, as compared to the uranium cycle, is a lower production of minor actinides, of which the radiological impact on the long term constitutes a problem. At present, nuclear data libraries don't provide cross sections of a good enough quality, allowing more realistic calculations from simulations related to these reactors. The {sup 232}Th neutron capture cross section is an example. With the n-TOF collaboration, the measurement of this reaction was achieved in 2002 using two C{sub 6}D{sub 6} detectors. The experimental area located at CERN, is characterized by an outstanding neutron energy resolution coupled to a high instantaneous neutron flux. The determination of the gamma-ray cascade detection efficiency, with a random behaviour, has been obtained by the use of weighting functions. These were deduced from Monte Carlo simulations with the code MCNP. Data extraction, reduction, and the description of the neutron flux have lead to the capture yield. In the resolved resonance region, the resonance parameters describing the cross section were deduced with the code SAMMY, using the R-matrix theory. In the unresolved resonance region, an uncertainty of 3,5% is found, and a comparison with recent measurements shows a good agreement. (author)

  14. Correction methodology for the spectral interfering {gamma}-rays overlapping to the analytical peaks used in the analysis of {sup 232}Th

    Energy Technology Data Exchange (ETDEWEB)

    Yuecel, H., E-mail: haluk.yucel@ankara.edu.t [Institute of Nuclear Sciences, Ankara University (Australia), Besevler Yerleskesi, Tandogan, 06100 Ankara (Turkey); Koese, E. [Institute of Nuclear Sciences, Ankara University (Australia), Besevler Yerleskesi, Tandogan, 06100 Ankara (Turkey); Esen, A.N. [Energy Institute, Istanbul Technical University (ITU), Maslak, 34469 Istanbul (Turkey); Bor, D. [Institute of Nuclear Sciences, Ankara University (Australia), Besevler Yerleskesi, Tandogan, 06100 Ankara (Turkey)

    2011-06-15

    In the {gamma}-ray spectrometric analysis of the radionuclides, a correction factor is generally required for the spectral interfering {gamma}-rays in determining the net areas of the analytical peaks because some interfering {gamma}-rays often might contribute to the analytical peaks of interest. In present study, a correction methodology for the spectral interfering {gamma}-rays (CSI) is described. In particular, in the analysis of {sup 232}Th contained in samples, the interfering {gamma}-rays due to {sup 226}Ra, {sup 235}U, {sup 238}U and their decay products often overlap to the peaks of interest from {sup 232}Th decay products, and vise versa. For the validation of the proposed CSI method, several certified reference materials (CRM) containing U and Th were measured by using a 76.5% efficient n-type Ge detector. The required correction factors were quantified for spectral interference, self-absorption and true coincidence summing (TCS) effects for the relevant {gamma}-rays. The measured results indicate that if one ignores the contributions of the interfering {gamma}-rays to the analytical peaks at 583.2 keV of {sup 208}Tl and 727.3 keV of {sup 212}Bi, this leads to a significantly systematic influence on the resulted activities of {sup 232}Th. The correction factors required for spectral interference and TCS effects are estimated to be {approx}13.6% and {approx}15.4% for 583.2 keV peak. For the 727.3 keV peak, the correction factor is estimated to be {approx}15% for spectral interference, and {approx}5% for the TCS effects at the presently used detection geometry. On the other hand, the measured results also indicate that ignoring the contribution of the interfering {gamma}-rays to the areas of the analytical peaks at 860.6 keV of {sup 208}Tl, 338.3 and 911.2 keV of {sup 228}Ac does not lead to any significant systematic influence on the {sup 232}Th analysis. Because these factors are remained generally less than {approx}5%, i.e., within overall uncertainty

  15. Use of radioactive methods for determination of uranium, neptunium, plutonium, americium and curium isotopes in waste radioactive; Utilizacao de metodos radioanaliticos para determinacao de isotopos de uranio, netunio, plutonio, americio e curio em rejeitos radioativos

    Energy Technology Data Exchange (ETDEWEB)

    Geraldo, Bianca

    2012-07-01

    Activated charcoal is a common type of radioactive waste that contains high concentrations of fission and activation products. The management of this waste includes its characterization aiming the determination and quantification of the specific radionuclides including those known as Difficult-to-Measure Radionuclides (RDM). The analysis of the RDM's generally involves complex radiochemical analysis for purification and separation of the radionuclides, which are expensive and time-consuming. The objective of this work was to define a methodology for sequential analysis of the isotopes of uranium, neptunium, plutonium, americium and curium present in a type of radioactive waste, evaluating chemical yield, analysis of time spent, amount of secondary waste generated and cost. Three methodologies were compared and validated that employ ion exchange (TI+EC), extraction chromatography (EC) and extraction with polymers (ECP). The waste chosen was the activated charcoal from the purification system of primary circuit water cooling the reactor IEA-R1. The charcoal samples were dissolved by acid digestion followed by purification and separation of isotopes with ion exchange resins, extraction and chromatographic extraction polymers. Isotopes were analyzed on an alpha spectrometer, equipped with surface barrier detectors. The chemical yields were satisfactory for the methods TI+EC and EC. ECP method was comparable with those methods only for uranium. Statistical analysis as well the analysis of time spent, amount of secondary waste generated and cost revealed that EC method is the most effective for identifying and quantifying U, Np, Pu, Am and Cm present in charcoal. (author)

  16. 230Th, 232Th and 238U determinations in phosphoric acid fertilizer and process products by ICP-MS

    International Nuclear Information System (INIS)

    Through processing of Santa Quiteria-CE mine phosphate rock, Brazil has established a project for production of phosphoric acid fertilizer and uranium as a by-product. Under leaching conditions of phosphate rock with sulfuric acid, which is the common route for preparing phosphoric acid fertilizer, a large part of uranium, thorium and their decay products naturally present in the rock are solubilized. In order to assess the contamination potential in phosphoric acid and others process products, this paper describes a previous precipitation and direct methods for routine analysis of thorium and uranium isotopes by ICP-MS. In all samples, 230Th, 232Th and 238U were directly determined after dilution, except 230Th in phosphoric acid loaded with uranium sample, which to overcome equipment contamination effect, was determined after its separation by oxalate precipitation using lanthanum as a carrier. The results obtained by the proposed method by ICP-MS, were in good agreement when compared to alpha spectrometry for 230Th, and ICP-OES and spectrophotometry with arsenazo III for elementary uranium and thorium determinations. (author)

  17. Analysis of radon, uranium 238 and thorium 232 in potable waters: Dose to adult members of the Moroccan urban population

    Science.gov (United States)

    Misdaq, M. A.; Ouabi, H.; Merzouki, A.

    2007-10-01

    Uranium (238U) and thorium (232Th) concentrations as well as radon (222Rn) and thoron (220Rn) alpha-activities per unit volume have been measured inside various potable water samples collected from nineteen cities in Morocco by using CR-39 and LR-115 type II solid state nuclear track detectors (SSNTDs). Measured radon alpha-activities ranged from (0.37 ± 0.02) Bq l-1 to (13.6 ± 1.10) Bq l-1 for the potable water samples studied. Alpha-activities due to radon from the ingestion of the studied potable water samples were determined in different compartments of the gastrointestinal system by using the ICRP compartmental model for radon. Annual committed equivalent doses due to radon were evaluated in the gastrointestinal compartments from the ingestion of the potable water samples studied. The influence of the target tissue mass, radon intake and alpha-activity integral due to radon on the annual committed equivalent doses in the gastrointestinal compartments was investigated.

  18. MApping the Most Massive Overdensities (MAMMOTH) II -- Discovery of an Extremely Massive Overdensity BOSS1441 at $z=2.32$

    CERN Document Server

    Cai, Zheng; Bian, Fuyan; Zabludoff, Ann; Yang, Yujin; Prochaska, J Xavier; McGreer, Ian; Zheng, Zhen-Ya; Kashikawa, Nobunari; Wang, Ran; Frye, Brenda; Green, Richard; Jiang, Linhua

    2016-01-01

    Cosmological simulations suggest a strong correlation between high optical-depth Ly$\\alpha$ absorbers, which arise from the intergalactic medium (IGM), and 3-D mass overdensities on scales of $10-30$ $h^{-1}$ comoving Mpc. By examining the absorption spectra of $\\sim$ 80,000 QSO sight-lines over a volume of 0.1 Gpc$^3$ in the Sloan Digital Sky Survey III (SDSS-III), we have identified an extreme overdensity, BOSS1441, which contains a rare group of strong Ly$\\alpha$ absorbers at $z=2.32\\pm 0.02$. This absorber group is associated with six QSOs at the same redshift on a 30 comoving Mpc scale. Using Mayall/MOSAIC narrowband and broadband imaging, we detect Ly$\\alpha$ emitters (LAEs) down to $0.7\\times L_{\\rm{Ly\\alpha}}^*$, and reveal a large-scale structure of Ly$\\alpha$ emitters (LAEs) in this field. Our follow-up Large Binocular Telescope (LBT) observations have spectroscopically confirmed 19 galaxies in the density peak. We show that BOSS1441 has an LAE overdensity of $10.8\\pm 2.6$ on a 15 comoving Mpc scale...

  19. A beta-alpha coincidence counting system for measurement of trace quantities of 238U and 232Th in aqueous samples at the Sudbury Neutrino Observatory.

    Science.gov (United States)

    Dawson, M.; Doucas, G.; Fergani, H.; Jelley, N. A.; Majerus, S.; O'Keeffe, H. M.; Peeters, S. J. M.; Perry, C.

    2016-08-01

    The Sudbury Neutrino Observatory experiment was built to measure the total flux of 8B solar neutrinos via the neutral current disintegration deuterium nuclei. This process can be mimiced by daughter isotopes of 232Th and 238U which can photodisintegrate the deuterium nucleus. Measurement of the concentration of such radioisotopes in the heavy water was critical to the success of the experiment. A radium assay technique using Hydrous Titanium Oxide coated filters was developed for this purpose and it was used in conjunction with a delayed beta-alpha coincidence counting system. The design, calibration and operation of this counting system are described in this paper. The counting efficiency for 232Th (224Ra) and 238U (226Ra) were measured to be 50 ± 5% and 62 ± 7%

  20. Distribution of radioactive pollution of 238U, 232Th, 40K and 137Cs in northwestern coasts of Persian Gulf, Iran

    International Nuclear Information System (INIS)

    A reconnaissance study has been made of the distribution of 238U, 232Th, 40K and 137Cs and geochemical features in soils and sediments samples at various locations in the northwestern coast of Persian Gulf. Activity concentration levels due to radionuclides were measured in 30 soil and sediment samples collected from this region. From the measured spectra, activity concentrations were determined for 40K (range from 146 to 500 Bq kg-1), 137Cs (from 5 to 20 Bq kg-1), 238U (from 21 to 65 Bq kg-1) and 232Th (from 15 to 45 Bq kg-1) with lowest limit detection (LLD) of 68, 3.2, 4.3 and 4.3 Bq kg-1, respectively. The dose rate from ambient air at the soil ranges was between 19 and 58 nGy h-1 with an average of 37.41 ± 9.66 nGy h-1

  1. Accelerated alpha-decay of 232U isotope achieved by exposure of its aqueous solution with gold nanoparticles to laser radiation

    CERN Document Server

    Simakin, A V

    2011-01-01

    Experimental results are presented on laser-induced accelerated alpha-decay of Uranium-232 nuclei under laser exposure of Au nanoparticles in aqueous solutions of its salt. It is demonstrated that the decrease of alpha-activity strongly depends on the peak intensity of the laser radiation in the liquid and is highest at several terawatt per square centimeter. The decrease of alpha-activity of the exposed solutions is accompanied by the deviation of gamma-activities of daughter nuclides of Uranium-232 from their equilibrium values. Possible mechanisms of the laser influence on the alpha-activity are discussed on the basis of the amplification of the electric field of laser wave on metallic nanoparticles.

  2. First reported incursion of highly pathogenic notifiable avian influenza A H5N1 viruses from clade 2.3.2 into European poultry.

    Science.gov (United States)

    Reid, S M; Shell, W M; Barboi, G; Onita, I; Turcitu, M; Cioranu, R; Marinova-Petkova, A; Goujgoulova, G; Webby, R J; Webster, R G; Russell, C; Slomka, M J; Hanna, A; Banks, J; Alton, B; Barrass, L; Irvine, R M; Brown, I H

    2011-02-01

    This study reports the first incursion into European poultry of H5N1 highly pathogenic notifiable avian influenza A (HPNAI) viruses from clade 2.3.2 that affected domestic poultry and wild birds in Romania and Bulgaria, respectively. Previous occurrences in Europe of HPNAI H5N1 in these avian populations have involved exclusively viruses from clade 2.2. This represents the most westerly spread of clade 2.3.2 viruses, which have shown an apparently expanding range of geographical dispersal since mid-2009 following confirmation of infections in wild waterfowl species in Mongolia and Eastern Russia. During March 2010, AI infection was suspected at post-mortem examination of two hens from two backyard flocks in Tulcea Country, Romania. HPNAI of H5N1 subtype was confirmed by reverse transcription polymerase chain reaction (RT-PCR). A second outbreak was confirmed 2 weeks later by RT-PCR, affecting all hens from another flock located 55 km east of the first cluster. On the same day, an H5N1 HPNAI virus was detected from a pooled tissue sample collected from a dead Common Buzzard found on the Black Sea coast in Bulgaria. Detailed genetic characterization of the haemagglutinin gene revealed the cleavage site of the isolates to be consistent with viruses of high pathogenicity belonging to clade 2.3.2 of the contemporary Eurasian H5N1 lineage. Viruses from a clade other than 2.2 have apparently spread to wild birds, with potential maintenance and spread through such populations. Whilst the scale of threat posed by the apparent westward spread of the clade 2.3.2 viruses remains uncertain, ongoing vigilance for clinical signs of disease as part of existing passive surveillance frameworks for AI, and the prompt reporting of suspect cases in poultry is advised.

  3. Isolation and lipid degradation profile of Raoultella planticola strain 232-2 capable of efficiently catabolizing edible oils under acidic conditions.

    Science.gov (United States)

    Sugimori, Daisuke; Watanabe, Mika; Utsue, Tomohiro

    2013-01-01

    The lipids (fats and oils) degradation capabilities of soil microorganisms were investigated for possible application in treatment of lipids-contaminated wastewater. We isolated a strain of the bacterium Raoultella planticola strain 232-2 that is capable of efficiently catabolizing lipids under acidic conditions such as in grease traps in restaurants and food processing plants. The strain 232-2 efficiently catabolized a mixture (mixed lipids) of commercial vegetable oil, lard, and beef tallow (1:1:1, w/w/w) at 20-35 °C, pH 3-9, and 1,000-5,000 ppm lipid content. Highly effective degradation rate was observed at 35 °C and pH 4.0, and the 24-h degradation rate was 62.5 ± 10.5 % for 3,000 ppm mixed lipids. The 24-h degradation rate for 3,000 ppm commercial vegetable oil, lard, beef tallow, mixed lipids, and oleic acid was 71.8 %, 58.7 %, 56.1 %, 55.3 ± 8.5 %, and 91.9 % at pH 4 and 30 °C, respectively. R. planticola NBRC14939 (type strain) was also able to efficiently catabolize the lipids after repeated subculturing. The composition of the culture medium strongly influenced the degradation efficiency, with yeast extract supporting more complete dissimilation than BactoPeptone or beef extract. The acid tolerance of strain 232-2 is proposed to result from neutralization of the culture medium by urease-mediated decomposition of urea to NH(3). The rate of lipids degradation increased with the rates of neutralization and cell growth. Efficient lipids degradation using strain 232-2 has been achieved in the batch treatment of a restaurant wastewater.

  4. Detection of VHE gamma-ray emission from the distant blazar 1ES 1101-232 with H.E.S.S. and broadband characterisation

    CERN Document Server

    Akhperjanian, A G; Beilicke, M; Benbow, W; Berge, D; Bernlöhr, K; Boisson, C; Bolz, O; Borrel, V; Braun, I; Brion, E; Brown, A M; Buhler, R; Büsching, I; Boutelier, T; Carrigan, S; Chadwick, P M; Chounet, L M; Coignet, G; Cornils, R; Costamante, L; Degrange, B; Dickinson, H J; Djannati-Atai, A; O'Connor-Drury, L; Dubus, G; Egberts, K; Emmanoulopoulos, D; Espigat, P; Farnier, C; Feinstein, F; Ferrero, E; Fiasson, A; Fontaine, G; Funk, Seb; Funk, S; Fussling, M; Gallant, Y A; Giebels, B; Glicenstein, J F; Glück, B; Goret, P; Hadjichristidis, C; Hauser, D; Hauser, M; Heinzelmann, G; Henri, G; Hermann, G; Hinton, J A; Hoffmann, A; Hofmann, W; Holleran, M; Hoppe, S; Horns, D; Jacholkowska, A; De Jager, O C; Kendziorra, E; Kerschhaggl, M; Khelifi, B; Komin, Nu; Kosack, K; Lamanna, G; Latham, I J; Le Gallou, R; Lemiere, A; Lemoine-Goumard, M; Lohse, T; Martin, J M; Martineau-Huynh, O; Marcowith, A; Masterson, C; Maurin, G; McComb, T J L; Moulin, E; De Naurois, Mathieu; Nedbal, D; Nolan, S J; Noutsos, A; Olive, J P; Orford, K J; Osborne, J L; Panter, M; Pelletier, G; Petrucci, P O; Pita, S; Pühlhofer, G; Punch, M; Ranchon, S; Raubenheimer, B C; Raue, M; Rayner, S M; Ripken, J; Rob, L; Rolland, L; Rosier-Lees, S; Rowell, G; Sahakian, V V; Santangelo, A; Sauge, L; Schlenker, S; Schlickeiser, R; Schroder, R; Schwanke, U; Schwarzburg, S; Schwemmer, S; Shalchi, A; Sol, H; Spangler, D; Spanier, F; Steenkamp, R; Stegmann, C; Superina, G; Tam, P H; Tavernet, J P; Terrier, R; Tluczykont, M; Van Eldik, C; Vasileiadis, G; Venter, C; Vialle, J P; Vincent, P; Völk, H J; Wagner, S J; Ward, M

    2007-01-01

    The blazar 1ES 1101-232 was observed with the High Energy Stereoscopic System (H.E.S.S.) of Atmospheric Cherenkov Telescopes (ACT) in 2004 and 2005, for a live time of 43 hours. VHE (E > 10^11 eV) gamma-rays were detected for the first time from this object. VHE observations of blazars are used to investigate the inner parts of the blazar jets, and also to study the extragalactic background light (EBL) in the near-infrared band. Observations in 2005 were conducted in a multiwavelength campaign, together with the RXTE satellite and optical observations. In 2004, simultaneous observations with XMM-Newton were obtained. 1ES 1101-232 was detected with H.E.S.S. with an excess of 722 photons, at a significance of 12 sigma. The measured VHE gamma-ray flux amounts to dN/dE = (5.63 +- 0.89) x 10^-13 (E/TeV)^-(2.94 +- 0.20) cm^-2 s^-1 TeV^-1, above a spectral energy threshold of 225 GeV. No significant variation of the VHE gamma-ray flux on any time scale was found. 1ES 1101-232 exhibits a very hard spectrum, and at a ...

  5. Distribution of 226Ra, 232Th, and 40K in rice plant components and physico-chemical effects of soil on their transportation to grains

    Directory of Open Access Journals (Sweden)

    Mohammed Saad Alsaffar

    2015-07-01

    Full Text Available Radioactivity distribution and transfer factor (TF in plants are crucial parameters used to assess radioactive contamination in the environment and its risks to humans. In this study, the activities of 226Ra, 232Th, and 40K were successfully measured via gamma-ray spectrometry on rice plant components (root, straw, husk, and grain and on corresponding soil samples collected from paddy fields in Penang, Malaysia. Soil physico-chemical characteristics (pH, cation exchange capacity, electrical conductivity, organic matter, and soil texture were also analyzed for their estimated effects on soil–grain TF. A major fraction of the total 226Ra and 232Th activities measured as 47% and 57%, respectively, were concentrated in the roots, whereas only about 9% and 8% were distributed in the grains, correspondingly. 40K activity accumulation was about 59% in the straw and 7% in the grains. Rice soil–grain TFs were observed in the ranges of (0.06–0.36 × 10−1 for 226Ra, (0.04–0.14 × 10−1 for 232Th, and (0.74–4.72 × 10−1 for 40K. Results showed that the selected radionuclide distributions in rice are dependent on component type, and their grain concentrations are not linearly related to their soil concentrations. These findings indicated that uptake predominantly depends on soil physico-chemical characteristics.

  6. Determination of {sup 228}Th, {sup 232}Th, and{sup 228}Ra in wild mushroom from a naturally high radioactive region in Brazil

    Energy Technology Data Exchange (ETDEWEB)

    Rosa, Mychelle M.L.; Taddei, Maria Helena T.; Silva, Marco A.; Ferreira, Marcelo T., E-mail: mychelle@cnen.gov.b, E-mail: mhtaddei@cnen.gov.b, E-mail: masilva@cnen.gov.b, E-mail: ferreira@cnen.gov.b [Brazilian Nuclear Energy Commission (LAPOC/CNEN-MG), Pocos de Caldas, MG (Brazil). Lab. of Pocos de Caldas; Maihara, Vera A., E-mail: vmaihara@ipen.gov.b [Nuclear and Energy Research Institute (IPEN/CNEN-SP), Sao Paulo, SP (Brazil)

    2011-07-01

    Mushrooms are fungi which efficiently accumulate radionuclides, as verified by radiochemistry analyses of specimens collected in contaminated areas, specifically after the Chernobyl nuclear accident. Many studies have demonstrated that mushrooms can be used in monitoring of ecosystem contamination and quality. The present paper is part of a broader study conducted in the Pocos de Caldas plateau region in Minas Gerais, Brazil, investigating assimilation of natural Uranium and Thorium radionuclide series by mushrooms. This region has elevated natural radioactivity due to the presence of radiological anomalies of volcanic origin. These anomalies are ore bodies containing Uranium and Thorium, the later being highly predominant. Many researchers have been conducted concerning radionuclide incorporation by agricultural products on the plateau. The present paper aims to determine {sup 232}Th, {sup 228}Th, and {sup 228}Ra radionuclides in wild mushrooms collected at different locations in the plateau region. {sup 228}Ra was determined by radiochemical separation using sulphate coprecipitation followed by beta radiometry. {sup 232}Th and {sup 228}Th were determined using anion exchange resin purification followed by alpha spectrometry. Higher values were obtained to {sup 228}Th than to {sup 232}Th. This is due to higher {sup 228}Ra mobility, which decays to {sup 228}Th. The accuracy of the analytical methods employed was evaluated using the reference sample IAEA Soil 327. These methods had high chemical recovery and high sensitivity. It was possible to confirm that mushrooms accumulate radionuclide and so can be used in environmental contamination and quality assessment. (author)

  7. Assay methods for U-238, Th-232, and Pb-210 in lead and calibration of Bi-210 bremsstrahlung emission from lead

    CERN Document Server

    Orrell, John L; Arnquist, Isaac J; Eggemeyer, Tere A; Glasgow, Brian D; Hoppe, Eric W; Keillor, Martin E; Morley, Shannon M; Myers, Allan W; Overman, Cory T; Shaff, Sarah M; Thommasson, Kimbrelle S

    2015-01-01

    Assay methods for measuring 238U, 232Th, and 210Pb concentrations in refined lead are presented. The 238U and 232Th concentrations are determined using isotope dilution inductively coupled plasma mass spectrometry (ID-ICP-MS) after anion exchange column separation of dissolved lead samples. The 210Pb concentration is inferred through {\\alpha}-spectroscopy of a daughter isotope, 210Po, after chemical precipitation separation on dissolved lead samples. Subsequent to the 210Po {\\alpha}-spectroscopy assay, a method for evaluating 210Pb concentrations in solid lead samples was developed via measurement of bremsstrahlung radiation from \\b{eta}-decay of a daughter isotope, 210Bi, by employing a 14-crystal array of high purity germanium (HPGe) detectors. Ten sources of refined lead were assayed. The 238U concentrations were <34 microBq/kg and the 232Th concentrations ranged <0.6-15 microBq/kg, as determined by the ICP-MS assay method. The 210Pb concentrations ranged from ~0.1-75 Bq/kg, as inferred by the 210Po ...

  8. Evaluation of Ra-226, Th-232 and K-40 activities concentrations and radium equivalent index in several Brazilian economic wall paints

    Energy Technology Data Exchange (ETDEWEB)

    Fonseca, Leandro M.; Pecequilo, Brigitte R.S., E-mail: lmfonseca@ipen.br, E-mail: brigitte@ipen.br [Instituto de Pesquisas Energeticas e Nucleares (IPEN/CNEN-SP), Sao Paulo, SP (Brazil)

    2015-07-01

    The titanium dioxide used as the white pigment in paints is produced from the processing of ilmenite minerals. As monazite, the main ilmenite radioactive contaminant, contains 1 to 20% thorium dioxide and also some uranium traces, so, eventually, wall paints can contain radioactivity. Activity concentrations of the naturally occurring radionuclides {sup 226}Ra, {sup 232}Th and {sup 40}K were determined in 15 Brazilian economic wall paints samples, by high resolution gamma-ray spectrometry. The activities concentrations in the studied samples ranged from 1.3 ± 0.2 Bq/kg to 23.4 ± 0.7 Bq/kg for {sup 226}Ra; from 2.5 ± 0.4 Bq/kg to 45.8 ± 1.5 Bq/kg for {sup 232}Th and from 5.8 ± 2.1 Bq/kg to 157 ± 22 Bq/kg for {sup 40}K. The radium equivalent index, calculated from the {sup 226}Ra, {sup 232}Th and {sup 40}K concentrations, varied from 1.30 Bq/kg up to 95.9 Bq/kg, below the value of 370 Bq/kg recommended by OECD for a safety use in residential building applications. (author)

  9. Determination of 238U, 232Th and 40K activity concentrations in riverbank soil along the Chao Phraya river basin in Thailand

    International Nuclear Information System (INIS)

    The activity concentrations of 238U, 232Th and 40K in riverbank soil along the Chao Phraya river basin was determined through gamma-ray spectrometry measurements made using a hyper-pure germanium detector in a low background configuration. The ranges of activity concentrations of 238U, 232Th and 40K were found to be 13.9 ↔ 76.8, 12.9 ↔ 142.9 and 178.4 ↔ 810.7 Bq kg−1, respectively. The anthropogenic radionuclide, 137Cs, was not observed in statistically significant amounts above the background level in the current study. The absorbed gamma dose rate in air at 1 m above the ground surface, the outdoor annual effective dose equivalent, the values of the radium equivalent activity and the external hazard index associated with all the soil samples in the present work were evaluated. The results indicate that the radiation hazard from primordial radionuclides in all soil samples from the area studied in this current work is not significant. - Highlights: • Radioactivity in surface soils from the Chao Phraya river basin in Thailand is evaluated. • Gamma-ray spectrometric analysis is to identify decays associated with 226Ra, 232Th and 40K. • The results provide baseline measurements for any changes in future radioactivity levels

  10. A preliminary study on 226Ra, 232Th, 40K and 137Cs activity concentrations in vegetables and fruits frequently consumed by inhabitants of Elazig Region, Turkey

    International Nuclear Information System (INIS)

    Determining radioactivity levels in foodstuffs is of great importance for the protection of human health. In addition, the literature includes few studies related to this subject in Turkey. In this study, gamma spectroscopic system was used in order to measure 226Ra, 232Th, 40K and 137Cs activity concentrations in vegetables and fruits produced in Elazig( Region. The average activity concentrations in vegetables was calculated as 0.64 ± 0.26 Bq kg-1 for 226Ra, 0.65 ± 0.14 Bq kg-1 for 232Th, 13.98 ± 1.22 Bq kg-1 for 40K, and 0.54 ± 0.04 Bq kg-1 for 137Cs. The average activity concentrations in fruits were 1.52 ± 0.34, 0.98 ± 0.23, 18.66 ± 1.13 and 0.59 ± 0.16 Bq kg-1, respectively for 226Ra, 232Th, 40K and 137Cs. Total committed effective dose value was determined as 20 and 30.55 μSv y-1, respectively for vegetables and fruits. The findings were compared with previous data reported for Turkey and other regions of the world. (author)

  11. Study of environmental natural gamma radiation dose and activity of uranium-238, thorium-232 using NaI (Tl) scintillation detector

    International Nuclear Information System (INIS)

    Exposure to ionizing radiation from natural sources is a continuous and unavoidable feature of life-systems on the earth. The environmental effective gamma radiation dose from terrestrial and cosmic radiation at height one foot above the earth's surface in open atmosphere has been measured at twenty different places in Sindhudurg district of Maharashtra state by using 2x2 NaI (Tl) scintillation detector. The activity of 238U and 232Th has been measured using gamma ray spectroscopy. The effective gamma radiation dose at different locations varies between, 0.286 to 0.804 mS/y, with an average value 0.512 mSv/y. The 238U activity varies from 0.466 KBq/m2 to 1.133 KBq/m2 with mean value of 0.684 KBq/m2. The 232Th activity varies from 0.552 KBq/m2 to 1.267 KBq/m2 with mean 0.8682 KBq/m2. The 238U to 232Th activity ratio varies from 0.494 to 1.47 with mean 0.898. (author)

  12. The Design Of RS-232 and RS-485 level converter based on the “master-slave”type device%“主-从”式装置的RS-232和RS-485电平转换器设计

    Institute of Scientific and Technical Information of China (English)

    钱玲玲

    2015-01-01

    At present, due to a low energy consumption, easy data management and maintenance, and other advantages,a master-slave device is widely used in industrial control systems,however,because the interface is not compatible with the level of the PC RS232 interface and the RS485 bus of the micro-controller,it need level conversion in order to achieve network link between them.Based on this,this paper introduced a RS485 interface chip SN75LBC184, and designed a low-cost,、good application RS232 / RS485 converter.%目前,主从式装置因具有系统能耗低、易于数据管理与维护等优势,而被广泛应用在工业控制系统中,但也因PC机的RS232接口与单片机的RS485总线的接口电平不兼容,要实现两者通信网络的链接需要进行电平转换。基于此,本文引入了一种RS485接口芯片STC11F02E,并设计了一种低成本、可靠性强、应用性能好的RS232/RS485转换器。

  13. Delayed Fission Gamma-ray Characteristics of Th-232 U-233 U-235 U-238 and Pu-239

    Energy Technology Data Exchange (ETDEWEB)

    Lane, Taylor [Sandia National Laboratories (SNL-NM), Albuquerque, NM (United States); Parma, Edward J. [Sandia National Laboratories (SNL-NM), Albuquerque, NM (United States)

    2015-08-01

    Delayed fission gamma-rays play an important role in determining the time dependent ioniz- ing dose for experiments in the central irradiation cavity of the Annular Core Research Reactor (ACRR). Delayed gamma-rays are produced from both fission product decay and from acti- vation of materials in the core, such as cladding and support structures. Knowing both the delayed gamma-ray emission rate and the time-dependent gamma-ray energy spectrum is nec- essary in order to properly determine the dose contributions from delayed fission gamma-rays. This information is especially important when attempting to deconvolute the time-dependent neutron, prompt gamma-ray, and delayed gamma-ray contribution to the response of a diamond photo-conducting diode (PCD) or fission chamber in time frames of milliseconds to seconds following a reactor pulse. This work focused on investigating delayed gamma-ray character- istics produced from fission products from thermal, fast, and high energy fission of Th-232, U-233, U-235, U-238, and Pu-239. This work uses a modified version of CINDER2008, a transmutation code developed at Los Alamos National Laboratory, to model time and energy dependent photon characteristics due to fission. This modified code adds the capability to track photon-induced transmutations, photo-fission, and the subsequent radiation caused by fission products due to photo-fission. The data is compared against previous work done with SNL- modified CINDER2008 [ 1 ] and experimental data [ 2 , 3 ] and other published literature, includ- ing ENDF/B-VII.1 [ 4 ]. The ability to produce a high-fidelity (7,428 group) energy-dependent photon fluence at various times post-fission can improve the delayed photon characterization for radiation effects tests at research reactors, as well as other applications.

  14. Synergy and antagonism of active constituents of ADAPT-232 on transcriptional level of metabolic regulation of isolated neuroglial cells.

    Directory of Open Access Journals (Sweden)

    Alexander George Panossian

    2013-02-01

    Full Text Available Gene expression profiling was performed on the human neuroglial cell line T98G after treatment with adaptogen ADAPT-232 and its constituents – extracts of Eleutherococcus senticosus root, Schisandra chinensis berry, and Rhodiola rosea root as well as several constituents individually, namely, eleutheroside E, schizandrin B, salidroside, triandrin, and tyrosol. A common feature for all tested adaptogens was their effect on G-protein-coupled receptor (GPCR signaling pathways, i.e. cAMP, phospholipase C and phosphatidylinositol signal transduction pathways. Adaptogens may reduce the cAMP level in brain cells by downregulation of adenylate cyclase gene ADC2Y and upregulation of phosphodiestherase gene PDE4D that is essential for energy homeostasis as well as for switching from catabolic to anabolic states and vice versa. All tested adaptogens up-regulated the PLCB1 gene, which encodes phosphoinositide-specific phospholipase C (PLC and phosphatidylinositol 3-kinases (PI3Ks, key players for the regulation of NF-B-mediated defense responses. Other common targets of adaptogens included genes encoding ERα estrogen receptor(2.9-22.6 fold down-regulation, cholesterol ester transfer protein (5.1-10.6 fold down-regulation, heat shock protein Hsp70 (3.0-45.0 fold up-regulation, serpin peptidase inhibitor (neuroserpin, and 5-HT3 receptor of serotonin (2.2-6.6 fold down-regulation. These findings can be reconciled with the observed beneficial effects of adaptogens in behavioral, mental and aging-associated disorders. Combining two or more active substances in one mixture significantly changes deregulated genes profiles: synergetic interactions result in activation of genes that none of the individual substances affected, while antagonistic interactions result in suppression some genes activated by individual substances. Merging of deregulated genes array profiles and intracellular networks is specific to the new substance with unique pharmacological

  15. Distribution of 226 Ra, 232 Th, 40 K and 137 Cs in soils of Province of Camaguey, Cuba

    International Nuclear Information System (INIS)

    A survey programme aimed at studying the environmental radioactivity in the Province of Camaguey in the eastern region of Cuba was undertaken. The average concentrations of 226 Ra, 232 Th, and 40 K in the surveyed soils were 26.4, 11.5 and 210 Bq.kg-1, respectively. The man-made radionuclide found was 137 Cs and its concentration was similar to those reported in regions affected only by global radioactive fallout, (7.9 Bq.kg-1). Radiological measurements carried out with a portable ionization chamber RSS-112 at the sampled sites revealed an average outdoor absorbed dose rate of 59.0 nGy.h-1 due to cosmic rays and terrestrial gamma radiation. Computed dose rates obtained through the UNSCEAR(1993) dose coefficients range from 4-182 nGy.h-1, with a mean value of 27.8 nGy.h-1, due to natural terrestrial gamma radiation. Ratio of Indoor to Outdoor absorbed dose rates in air was 1.75. The average value of absorbed dose rate in air for the ionizing component of cosmic rays was 31.8 nGy.h-1 at sea level. Because of the 95% of the Camaguey population lives at altitudes close to sea level (10-100 m), the absorbed dose rate in outdoor air from ionizing component of cosmic rays was estimated to be 32.3 nGy.h-1. An annual average effective dose equivalent of 510 μSv was estimated for Camaguey population due to the ionizing component of cosmic and gamma terrestrial radiation. This value is lower than the 760 μSv.year-1 estimated as a world average by UNSCEAR (1993). (author)

  16. Physical and underway data collected aboard the THOMAS G. THOMPSON during cruise TN232 in the Philippine Sea from 2009-04-02 to 2009-04-17 (NODC Accession 0104350)

    Data.gov (United States)

    National Oceanic and Atmospheric Administration, Department of Commerce — NODC Accession 0104350 includes physical and underway data collected aboard the THOMAS G. THOMPSON during cruise TN232 in the Philippine Sea from 2009-04-02 to...

  17. Comment: 232 [Taxonomy Icon

    Lifescience Database Archive (English)

    Full Text Available 2.png Hideko Urushihara (University of Tsukuba) licensed under CC Attribution2.1 Japan 写真提供:漆原秀子 (筑波大学) Phot...ograph provided by Hideko Urushihara (University of Tsukuba) bando 2010/08/04 09:34:37 2010/08/04 09:45:33 ...

  18. Solubility and speciation studies of waste radionuclides pertinent to geologic disposal at Yucca Mountain: Results on neptunium, plutonium and americium in J-13 groundwater; Letter report (R707): Reporting period, October 1, 1985--September 30, 1987

    Energy Technology Data Exchange (ETDEWEB)

    Nitsche, H.; Standifer, E.M.; Lee, S.C.; Gatti, R.C.; Tucker, D.B.

    1988-01-01

    We have studied the solubilities of neptunium, plutonium, and americium in J-13 groundwater from Yucca Mountain (Nevada) at three temperatures and hydrogen ion concentrations. They are 25{degree}, 60{degree}C, and 90{degree}C and pH 5.9, 7.0, and 8.5. The results for 25{degree}C are from a study which we did during FY 1984. We included these previous results in the tables to give more information on the solubility temperature dependence; they were, however, done at only one pH (7.0). The solubilities were studied from oversaturation. The nuclides were added at the beginning of each experiment as NpO{sub 2}{sup +}, Pu{sup 4+}, and Am{sup 3+}. The neptunium solubility decreased with increasing temperature and with increasing pH. The soluble neptunium did not change oxidation state at steady state. The pentavalent neptunium was increasingly complexed by carbonate with increasing pH. All solids were crystalline and contained carbonate, except the solid formed at 90{degree}C and pH 5.9. We identified this solid as crystalline Np{sub 2}P{sub 5}. The 25{degree}C, pH 7 solid was Na{sub 3}NpO{sub 2}(CO{sub 3}){sub 2} {center_dot} nH{sub 2}O. Plutonium concentrations decreased with increasing temperature and showed no trend with pH. Pu(V) and Pu(VI) were the dominant oxidation states in the supernatant solution; as the amount of Pu(V) increased with pH, Pu(VI) decreed. The steady-state solids were mostly amorphous, although some contained a crystalline component. They contained Pu(IV) polymer and unknown carbonates.

  19. Radiation protection - radionuclides - Synthesis sheets: Thorium-232 (ED 4317), Gallium-67 (ED 4314), Indium-111 (ED 4315), Chromium-51 (ED 4313), Thallium-201 (ED 4312), Phosphorus-33 (ED 4316), Fluorine- 18 (ED 4311), Yttrium-90 (ED 4310), Americium-241 (ED 4308), Strontium-90 (ED 4309), Sulfur-35 (ED 4307), Iodine-125 (ED 4306), Phosphorus-32 (ED 4305), Iodine-123 (ED 4304), Tritium (ED 4303), Carbon-14 (ED 4302), Technetium-99m (ED 4301), Iodine-131 (ED 4300)

    International Nuclear Information System (INIS)

    For each radionuclide, this document presents its characteristics (origin, radio-physical properties, biological properties), gives an overview of its uses, indicates and discusses its dosimetric parameters (for internal or external exposure), indicates radiation detection and contamination measurement techniques, gives an overview of means of protection (for premises, against external or internal exposure), describes the delimitation and control of premises, describes aspects related to personnel classification, training and medical monitoring, comments the issue of effluents and wastes, indicates administrative procedures related to the authorization and declaration of possession and use of sealed and unsealed sources, addresses the issue of transport, and describes what is to be done in case of incident or accident

  20. {sup 238}U and {sup 232}Th concentrations in various foodstuffs in Morocco and resulting radiation doses to the members of the public; Concentrations en {sup 238}U et {sup 232}Th dans differents aliments au Maroc et doses de radiations en resultant pour les membres du public

    Energy Technology Data Exchange (ETDEWEB)

    Misdaq, M.A.; Elamyn, H.; Erramli, H. [Cadi Ayyad Univ., Nuclear Physics and Techniques Lab., Faculty of Sciences Semlalia, Marrakech (Morocco)

    2008-04-15

    Uranium ({sup 238}U) and thorium ({sup 232}Th) concentrations were measured in different foods widely consumed in Morocco by using C.R.-39 and L.R.-115 type II solid state nuclear track detectors (S.S.N.T.D.). Data obtained were compared to those obtained by using isotope dilution mass spectrometry (I.D.M.S.). Total daily intakes of {sup 238}U and {sup 232}Th for a typical food basket were estimated to be 1.3 {+-} 0.1 mBq d{sup -1} and 0.98 {+-} 0.08 mBq d{sup -1}, 1.4 {+-} 0.1 mBq d{sup -1} and 1.06 {+-} 0.08 mBq d{sup -1}, 1.7 {+-} 0.1 mBq d{sup -1} and 1.26 {+-} 0.08 mBq d{sup -1} and 2.0 {+-} 0.1 mBq d{sup -1} and 1.5 {+-} 0.1 Bq d{sup -1} for the 2-7 years, 7-12 years, 12-17 years and adult's age groups, respectively. Alpha-activities due to annual {sup 238}U and {sup 232}Th intakes from the ingestion of the studied foodstuffs were determined in different organs and tissues of the human body of members of the public by using the ICRP gastrointestinal tract and systemic part models for these radionuclides. Committed equivalent doses due to annual intakes of {sup 238}U and {sup 232}Th were evaluated in the human body organs and tissues for different age groups of the Moroccan population by exploiting data obtained for alpha-doses deposited by 1 Bq of {sup 238}U and 1 Bq of {sup 232}Th in the considered human organs and tissues. The influence of the mass of the target tissue and activities due to {sup 238}U and {sup 232}Th on the committed equivalent doses due to annual intakes of these radionuclides in the organs and tissues of the human body was studied. (authors)

  1. Studies of TBX4 and chromosome 17q23.1q23.2: an uncommon cause of nonsyndromic clubfoot

    Science.gov (United States)

    Lu, W.; Bacino, C. A.; Richards, B.S.; Alvarez, C.; VanderMeer, J.E.; Vella, M.; Ahituv, N.; Sikka, N.; Dietz, F.R.; Blanton, S.H.; Hecht, J.T.

    2012-01-01

    Clubfoot is a common birth defect characterized by inward posturing and rigid downward displacement of one or both feet. The etiology of syndromic forms of clubfoot is varied and the causes of isolated clubfoot are not well understood. A microduplication of 2.2 Mb on chromosome 17q23.1q23.2 which includes T-box 4 (TBX4), a hindlimb-specific gene, and 16 other genes was recently identified in 3 of 66 families reported as nonsyndromic clubfoot, but additional non-foot malformations place them in the syndromic clubfoot category. Our study assesses whether variation in or around TBX4 contributes to nonsyndromic clubfoot. To determine whether this microduplication was a common cause of nonsyndromic clubfoot, 605 probands (from 148 multiplex and 457 simplex families) with nonsyndromic clubfoot were evaluated by copy number and oligonucleotide array CGH testing modalities. Only one multiplex family (0.68%) that had 16 with clubfoot and 9 with other foot anomalies, had a 350kb microduplication, which included the complete duplication of TBX4 and NACA2 and partial duplication of BRIP1. The microduplication was transmitted in an autosomal dominant pattern and all with the microduplication had a range of phenotypes from short wide feet and toes to bilateral clubfoot. Minimal evidence was found for an association between TBX4 and clubfoot and no pathogenic sequence variants were identified in the two known TBX4 hindlimb enhancer elements. Altogether, these results demonstrate that variation in and around the TBX4 gene and the 17q23.1q23.2 microduplication are not a frequent cause of this common orthopedic birth defect and narrows the 17q23.1q23.2 nonsyndromic clubfoot-associated region. PMID:22678995

  2. Impact of Chisan (ADAPT-232) on the quality-of-life and its efficacy as an adjuvant in the treatment of acute non-specific pneumonia.

    Science.gov (United States)

    Narimanian, M; Badalyan, M; Panosyan, V; Gabrielyan, E; Panossian, A; Wikman, G; Wagner, H

    2005-11-01

    A double-blind, placebo-controlled, randomized (simple randomisation), pilot (phase III) study of Chisan, (ADAPT-232; a standardised fixed combination of extracts of Rhodiola rosea L., Schisandra chinensis Turcz. Baill., and Eleutherococcus senticosus Maxim) was carried out on two parallel groups of patients suffering from acute nonspecific pneumonia. Sixty patients (males and females; 18-65 years old) received a standard treatment with cephazoline, bromhexine, and theophylline: in addition, one group of 30 patients was given Chisan mixture, whilst the second group of 30 patients received a placebo, each medication being taken twice daily from the beginning of the study for 10-15 days. The primary outcome measurements were the duration of antibiotic therapy associated with the clinical manifestations of the acute phase of the disease, together with an evaluation of mental performance in a psychometric test and the self-evaluation of quality-of-life (QOL) (WHOQOL-Bref questionnaires) before treatment and on the first and fifth days after clinical convalescence. The mean duration of treatment with antibiotics required to bring about recovery from the acute phase of the disease was 2 days shorter in patients treated with Chisan compared with those in the placebo group. With respect to all QOL domains (physical, psychological, social and ecological), patients in the Chisan group scored higher at the beginning of the rehabilitation period, and significantly higher on the fifth day after clinical convalescence, than patients in the control group. Clearly, adjuvant therapy with ADAPT-232 has a positive effect on the recovery of patients by decreasing the duration of the acute phase of the illness, by increasing mental performance of patients in the rehabilitation period, and by improving their QOL. Both the clinical and laboratory results of the present study suggest that Chisan (ADAPT-232) can be recommended in the standard treatment of patients with acute non

  3. A Hard X-ray View on Two Distant VHE Blazars: 1ES 1101-232 and 1ES 1553+113

    Energy Technology Data Exchange (ETDEWEB)

    Reimer, A.; Costamente, L.; /Stanford U., HEPL /KIPAC, Menlo Park; Madejski, G.; /KIPAC, Menlo Park /SLAC; Reimer, O.; /Stanford U., HEPL /KIPAC, Menlo Park; Dorner, D.; /Wurzburg U.

    2008-05-02

    TeV-blazars are known as prominent non-thermal emitters across the entire electromagnetic spectrum with their photon power peaking in the X-ray and TeV-band. If distant, absorption of -ray photons by the extragalactic background light (EBL) alters the intrinsic TeV spectral shape, thereby affecting the overall interpretation. Suzaku observations for two of the more distant TeV-blazars known to date, 1ES 1101-232 and 1ES 1553+113, were carried out in May and July 2006, respectively, including a quasi-simultaneous coverage with the state of the art Cherenkov telescope facilities. We report on the resulting data sets with emphasis on the X-ray band, and set into context to their historical behavior. During our campaign, we did not detect any significant X-ray or {gamma}-ray variability. 1ES 1101-232 was found in a quiescent state with the lowest X-ray flux ever measured. The combined XIS and HXD PIN data for 1ES 1101-232 and 1ES 1553+113 clearly indicate spectral curvature up to the highest hard X-ray data point ({approx} 30 keV), manifesting as softening with increasing energy. We describe this spectral shape by either a broken power law or a log-parabolic fit with equal statistical goodness of fits. The combined 1ES 1553+113 very high energy spectrum (90-500 GeV) did not show any significant changes with respect to earlier observations. The resulting contemporaneous broadband spectral energy distributions of both TeV-blazars are discussed in view of implications for intrinsic blazar parameter values, taking into account the {gamma}-ray absorption in the EBL.

  4. Determination of radioactivity level of 238U, 232Th and 40K in surface medium in Zhuhai city by in-situ gamma-ray spectrometry

    International Nuclear Information System (INIS)

    A gamma-ray spectrometry survey with NaI(Tl) (φ75mm x 75mm) has been performed on a large scale to determine the distribution of 40K, 238U and 232Th in soil and rocks in Zhuhai, a southern Chinese city located in Guangdong Province. The survey sampled 970 sites which covered an area of more than 100 km2. The average activities of 40K. 238U and 222Th were found 655±338, 85.8±31.6, and 159.8±49.0 Bq·kg-1 in soil or cement of pavement in the urban area; 832±455, 87.3±41.6, and 179.3±40.7 Bq·kg-1 in weathered granite; 634±76.8, 35.2±14.6 and 70.2±18.6Bq·kg-1 in the Quaternary sediments in Doumen District. The average 232Th activity (159.8±49.0 Bq·kg-1) is above the average in both China (49 Bq·kg-1) and the world (30 Bq·kg-1). Terrestrial air-absorbed dose rates calculated from the above activities are 85.08±15.63, 183.33±40.80 nGy·h-1 respectively over the Quaternary sediments and weathered granite, and 163.49±30.15 nGy·h-1 in the urban area. The average calculated air-absorbed dose rate is about 12.63% larger than the value measured by a portable plastic scintillator dosemeter. The 40K, 238U and 232Th activities in surface medium are mainly originated from biotite granites, as indicated by a strong correlation between the radioactivity level and geological lithology in the surveyed area. (author)

  5. Fusion hybrids for generation of advanced (231Pa+232U+233U+234U)-fuel in closed (U-Pu-Th)-fuel cycle

    International Nuclear Information System (INIS)

    Technology of controlled thermonuclear fusion (CTF) is traditionally regarded as a practically inexhaustible energy source. However, development, mastering, broad deployment of fast breeder reactors and closure of nuclear fuel cycle (NFC) can also extend fuel base of nuclear power industry (NPI) up to practically unlimited scales. Under these conditions, it seems reasonable to introduce into a circle of the CTF-related studies the works directed towards solving some principal problems which can appear in a large-scale NPI in closed NFC. The first challenge is a large scale of operations in NFC back-end that should be reduced by achieving substantially higher fuel burn-up in power nuclear reactors. The use of 231Pa-232Th-232U-233U fuel in light-water reactor (LWR) opens a possibility of principle to reach very high (about 30% HM) or even ultra-high fuel burn-up. The second challenge is a potential unauthorized proliferation of fissionable materials. As is known, a certain remarkable quantity of 232U being introduced into uranium fraction of nuclear fuel can produce a serious barrier against switching the fuel over to non-energy purposes. Involvement of hybrid thermonuclear reactors (HTR) into NPI structure can substantially facilitate resolving these problems. If HTR will be involved into NPI structure, then main HTR mission consists not in energy generation but in production of nuclear fuel with a certain isotope composition. The present paper analyzes some neutron-physical features in production of advanced nuclear fuels in thorium HTR blankets. The obtained results demonstrated that such a nuclear fuel may be characterized by very stable neutron-multiplying properties during full LWR operation cycle and by enhanced proliferation resistance too. The paper evaluates potential benefits from involvement of HTR with thorium blanket into the international closed NFC. (author)

  6. Quantification of transfer of {sup 238}U, {sup 226}Ra, {sup 232}Th, {sup 40}K and {sup 137}Cs in mosses of a semi-natural ecosystem

    Energy Technology Data Exchange (ETDEWEB)

    Dragovic, S., E-mail: sdragovic@inep.co.r [Institute for the Application of Nuclear Energy - INEP, University of Belgrade, Banatska 31b, 11080 Belgrade (Serbia); Mihailovic, N. [Institute for the Application of Nuclear Energy - INEP, University of Belgrade, Banatska 31b, 11080 Belgrade (Serbia); Gajic, B. [Faculty of Agriculture, Institute of Land Management, Laboratory of Soil Physics, University of Belgrade, Nemanjina 6, 11081 Belgrade (Serbia)

    2010-02-15

    There is a lack of appropriate data on transfer of some radionuclides on many terrestrial biota groups. To expand the available data concentration ratios of {sup 238}U, {sup 226}Ra, {sup 232}Th, {sup 40}K and {sup 137}Cs in mosses are presented in this paper. The relationship between concentration ratios of radionuclides and physicochemical characteristics of the underlying soil was also investigated. The data on concentration ratios obtained here will provide a useful addition to the currently used database of transfer parameters, particularly for natural radionuclides.

  7. Analysis of 226Ra, 232Th 40К and 137Cs in samples of soil from some areas of Republic of Macedonia by using gamma spectrometry

    Directory of Open Access Journals (Sweden)

    Todorovik Aleksandra

    2012-01-01

    Full Text Available Taking into consideration the importance of the distribution and transfer of radio nuclides in soil, an attempt was made in this work to determine the concentration of 226Ra, 232Th 40К and 137Cs in the same. The concentrations of activity in the gamma-absorbed dose rates of the terrestrial naturally occurring radio nuclides, as follows, 226Ra, 232Th and 40K were determined in samples of soil collected from some parts of Republic of Macedonia, i.e. from three major cities in the Republic of Macedonia. The samples are taken by means of a special dosage dispenser which enables sampling of samples at a depth of 0-5 cm, 5-10cm and 10-15cm, thus disabling the sampling above these layers of soil. An identification of radio nuclides and assessment of their activity has been performed by applying gamma spectrometry. The time of counting for each sample was 65000 s. in order to obtain statistically small mistake. The spectrums were analyzed by a commercially available software GENIE-2000 received from Canberra, Austria. The activity of soil had wide range of values: 20.3 to 82.9 Bq kg-1for 226Ra, 16.1 to 82.5 Bq kg-1 for 232Th, 325 to 799.0 Bq kg-1for 40К and 9.1 to 24.3 Bq kg-1for 137Cs, respectively. The concentrations of these radio nuclides have been compared with the available data from the other countries. Natural environmental radioactivity and the associated external exposure due to gamma radiation depend primarily on the geological and geographical conditions. Namely, the specific levels of terrestrial environmental radiation are related to the type of rocks from which the soils originate. The obtained data indicate that the average value of activity of 232Th is about higher than the one of 226Ra The concentration of activity of 40К in the soil has greater value than 32Th and 226Ra in all soils. The causes for the existence of 137Cs in these soils are the nuclear explosions, waste radioactive materials and other incidents. It reaches the

  8. CSER 90-006, addendum 1: Criticality safety control for source term reduction project in the scrubber glovebox of Building 232-Z. Revision 1

    International Nuclear Information System (INIS)

    This Criticality Safety Evaluation Report addendum extends the coverage of the original CSER (90-006) about dismantling the ductwork in 232-Z to include cleanout of the Scrubber Glovebox, with an estimated residual Pu holdup of less than 200 grams. For conservatism and containment considerations, the provisions about waste packaging and water exclusion from the original work are retained, even though it is not credible for the Scrubber Pu content to be made critical with water added (NDA gives about 1/3 a minimum critical mass)

  9. Neutron capture cross section of $^{232}Th$ measured at the nTOF facility at CERN in the unresolved resonance region up to 1 MeV

    CERN Document Server

    Aerts, G; Alvarez, H; Alvarez-Velarde, F; Andriamonje, Samuel A; Andrzejewski, J; Assimakopoulos, P A; Audouin, L; Badurek, G; Baumann, P; Becvar, F; Berthoumieux, E; Calviño, F; Cano-Ott, D; Capote, R; Carillo de Albornoz, A; Cennini, P; Chepel, V Yu; Chiaveri, Enrico; Colonna, N; Cortés, G; Couture, A; Cox, J; Dahlfors, M; David, S; Dillman, I; Dolfini, R; Domingo-Pardo, C; Dridi, W; Durán, I; Eleftheriadis, C; Embid-Segura, M; Ferrant, L; Ferrari, A; Ferreira-Marques, R; Fitzpatrick, L; Frais-Kölbl, H; Fujii, K; Furman, W; Gonçalves, I; González-Romero, E M; Goverdovski, A; Gramegna, F; Griesmayer, E; Guerrero, C; Gunsing, F; Haas, B; Haight, R; Heil, M; Herrera-Martínez, A; Igashira, M; Isaev, S; Jericha, E; Käppeler, F K; Kadi, Y; Karadimos, D; Karamanis, D; Kerveno, M; Ketlerov, V; Köhler, P; Konovalov, V; Kossionides, E; Krticka, M; Lamboudis, C; Leeb, H; Lindote, A; Lopes, I; Lozano, M; Lukic, S; Marganiec, J; Marques, L; Marrone, S; Mastinu, P; Mengoni, A; Milazzo, P M; Moreau, C; Mosconi, M; Neves, F; Oberhummer, Heinz; O'Brien, S; Oshima, M; Pancin, J; Papachristodoulou, C; Papadopoulos, C; Paradela, C; Patronis, N; Pavlik, A; Pavlopoulos, P; Perrot, L; Pigni, M T; Plag, R; Plompen, A; Plukis, A; Poch, A; Pretel, C; Quesada, J; Rauscher, T; Reifarth, R; Rosetti, M; Rubbia, Carlo; Rudolf, G; Rullhusen, P; Salgado, J; Sarchiapone, L; Savvidis, I; Stéphan, C; Taliente, G; Taín, J L; Tassan-Got, L; Tavora, L; Terlizzi, R; Vannini, G; Vaz, P; Ventura, A; Villamarín, D; Vincente, M C; Vlachoudis, V; Vlastou, R; Voss, F; Walter, S; Wendler, H; Wiescher, M; Wisshak, K

    2006-01-01

    We have measured the neutron capture reaction yield of /sup 232energy range from 1 eV to 1 MeV. The average capture cross section has been extracted in the energy range from 4 keV up to 1 MeV with an overall accuracy better than 4%. An independent IAEA evaluation shows good agreement with the data. The average cross section has been expressed in terms of average resonance parameters using the partial waves script l=0,1, and 2.

  10. Comparison of the (p,xn) cross sections from /sup 238/U, /sup 235/U, and /sup 232/Th targets irradiated with 200-MeV protons

    Energy Technology Data Exchange (ETDEWEB)

    Chu, Y.Y.; Zhou, M.L.

    1982-01-01

    We have measured absolute cross sections for (p,xn) reactions (x ranges from 0 to 8) from /sup 238/U, /sup 235/U, and /sup 232/Th targets irradiated with 200-MeV protons at the Brookhaven AGS Linac injector. Chemical yields were determined by using /sup 239/Np and /sup 233/Pa as tracers. Yield patterns obtained in this work can be compared to the experimental results and theoretical calculations from earlier work, and they are consistent within the framework of intranuclear cascade followed by neutron evaporation and fission competition.

  11. Daily intake of /sup 234,235,238/U, /sup 228,230,232/Th and /sup 226,228/Ra by New York City residents

    International Nuclear Information System (INIS)

    The daily intake of long-lived alpha-emitting members of the U, Th and Ac series by New York City residents has been estimated from measurements of diet, water and air samples. The total daily intakes from inhalation, food and water consumption in mBq are 18 (234U), 0.7 (235U), 16 (238U), 6 (230Th), 4 (232Th) and 52 (226Ra). From this, we infer that the total daily intakes of 228Th and 228Ra are 4 and 35 mBq, respectively

  12. Cost-based optimizations of power density and target-blanket modularity for {sup 232}Th/{sup 233}U-based ADEP

    Energy Technology Data Exchange (ETDEWEB)

    Krakowski, R.A.

    1995-07-01

    A cost-based parametric systems model is developed for an Accelerator-Driven Energy Production (ADEP) system based on a {sup 232}Th/{sup 233}U fuel cycle and a molten-salt (LiF/BeF{sub 2}/ThF{sub 3}) fluid-fuel primary system. Simplified neutron-balance, accelerator, reactor-core, chemical-processing, and balance-of-plant models are combined parametrically with a simplified costing model. The main focus of this model is to examine trade offs related to fission power density, reactor-core modularity, {sup 233}U breeding rate, and fission product transmutation capacity.

  13. Methods for the determination of 234U/230 U, 230Th/232 Th and 228Ra/226Ra in uranium ores by TIMS%TIMS测定铀矿石样品中234U/238U、230Th/232Th、228Ra/226Ra的方法研究

    Institute of Scientific and Technical Information of China (English)

    朱明燕; 郭冬发; 崔建勇; 刘宇昂; 谭靖; 张彦辉

    2009-01-01

    研究了TIMS测定铀矿石样品中234 U/238 U、230 Th/232 Th、228 Ra/226 Ra的方法.建立了铀矿石密闭混酸一次溶样的方法和采用阴离子、阳离子和Sr特效树脂逐级离子交换分离纯化U、Th和Ra的流程,满足了TIMS测量要求.测定结果表明:100~1000 ng的天然铀中234U/238U,其测量精密度从静态多接收的2.34%提高到动态多接收的0.47%;对230Th与232Th丰度接近、质量为1 μg左右的钍,采用三带点样技术和法拉第多接收技术测定230Th/232Th,其内精度平均值为0.0048%,外精度为0.028%;采用单带加钽发射剂,ETP跳峰测定50~100 fg镭-228稀释剂中的228Ra/226Ra,其内精度小于0.10%,外精度小于0.20%.比较TIMS和HR-ICP-MS、α能谱法测定234U/238U、230Th/232Th、228Ra/226Ra结果,三者结果相吻合.TIMS测量法样品用量少、快速、准确、精密度高,是U,Th、Ra同位素比值测定方法的又一补充.

  14. Fission Cross-Section Measurements of the Odd-Odd Isotopes 232Pa, 238Np, and 236Np

    Energy Technology Data Exchange (ETDEWEB)

    Danon, Y. [Rensselaer Polytechnic Institute; Moore, M. S. [Los Alamos National Laboratory (LANL); Koehler, Paul Edward [ORNL; Littleton, P. E. [Los Alamos National Laboratory (LANL); Miller, G. G. [Los Alamos National Laboratory (LANL); Ott, M. A. [Los Alamos National Laboratory (LANL); Rowton, L. J. [Los Alamos National Laboratory (LANL); Taylor, W. A. [Los Alamos National Laboratory (LANL); Wilhelmy, J. B. [Los Alamos National Laboratory (LANL); Yates, M. A. [Los Alamos National Laboratory (LANL); Carlson, A. D. [National Institute of Standards and Technology (NIST); Hill, Nathaniel [ORNL; Harper, R. [EG& G Energy Measurements, Los Alamos, NM; Hilko, R. [EG& G Energy Measurements, Los Alamos, NM

    1996-01-01

    Transmutation of actinide waste into fission products could be enhanced by using resonance fission of odd-odd target materials; those of interest are 232Pa, 238Np, and 242Am. Fission cross-section measurements of two of these short-lived materials were performed at Los Alamos National Laboratory. Samples were produced by the (d,2n) reaction in the Los Alamos Ion Beam Facility followed by fast radiochemistry to separate the odd-odd target of interest. The fission cross section of the nanogram samples was measured in a high intensity pulsed neutron beam produced by 800-MeV proton spallation. Using this procedure, the fission cross sections of the 1.3-day 232Pa and 2.1-day 238Np were successfully measured in the energy range from 0.01 eV to 50 keV. The fission cross section of the relatively long-life isotope 236Np was also measured in the same system while the short half-life isotopes were being prepared. The results and resonance analysis are presented.

  15. Estimation of dose contribution from 226Ra, 232Th and 40K radon exhalation rates in soil samples from Shivalik foot hills in India.

    Science.gov (United States)

    Chauhan, R P; Chauhan, Pooja; Pundir, Anil; Kamboj, Sunil; Bansal, Vakul; Saini, R S

    2014-01-01

    The concentration of radium, thorium and potassium and radon exhalation rates in soil samples collected from Shivalik foot hills in the states of Haryana and Himachal Pradesh (India) were experimentally measured. A high-resolution gamma-ray spectroscopic system was used for the measurement of natural radioactivity ((226)Ra, (232)Th and (40)K) at Inter-University Accelerator Center, New Delhi, using a coaxial n-type high-purity germanium detector (EG&G, ORTEC, Oak Ridge, USA). The mass exhalation rates (EM) of radon in soil samples from the study area measured by 'sealed canister technique' using LR-115 type II track detectors varied from 50±1 to 143±6 mBqkg(-1) h(-1). The activity concentrations of (226)Ra, (232)Th and (40)K in various soil samples of the study area varied from 31±1.3 to 63±4.6, 53±1.8 to 78±2.6 and 472±4.8 to 630±7.0 Bq kg(-1) respectively. The results indicated some higher levels of radioactivity in Lal Dhang peak area of the hills compared with other locations under study. PMID:23893776

  16. Distribution of 238U, 232Th, 40K, and 137Cs concentrations in soil samples nearby a nuclear laboratory, Capao Island, Brazil

    Directory of Open Access Journals (Sweden)

    Oliveira Luciano S.R.

    2015-01-01

    Full Text Available Absolute soil concentrations of 238U, 232Th, 40K, and 137Cs samples were measured using high-resolution gamma spectrometry. The area of interest encompasses an embankment in a mangrove swamp in Guaratiba, Rio de Janeiro, called Capao Island, where nuclear, chemical and biological defense laboratories of the Brazilian Army Technology Center are in operation for more than 30 years. In order to ensure that no significant environmental impact has resulted from neutron physics experiments performed in a graphite exponential pile in addition to the operation of two cesium-driven irradiating facilities, radiation monitoring of the isotopes was carried out. A total of eight 250 ml soil samples were extracted within an area of 300 m x 300 m. No trace of 137Cs was detected and the measured levels of 238U were found to be close to the global mean. However, some data that slightly exceeded the expected normal range for 232Th (60 % of samples and 40K (20 % of samples should be attributed to the construction debris (cement, rocks, and sand used in the embankment at the site. Since there is no handling of those isotopes at that site or adjacent facilities that could affect their presence, it was concluded that no detectable contamination has occurred.

  17. Measurement of double-differential neutron emission cross sections of 238U, 232Th and 12C for 18 MeV neutrons

    International Nuclear Information System (INIS)

    Double-differential neutron emission cross sections of 238U, 232Th and 12C have been measured for 18-MeV incident neutrons using the neutron time-of-flight technique and Tohoku University 4.5MV Dynamitron accelerator as a pulsed neutron generator. In the experiment, energy resolution of the spectrometer was improved by employing a newly developed post-acceleration beam-chopper and by adjustment of timing property of the neutron detector. Measurements were made at laboratory angles between 30- and 145- deg., and data were obtained for secondary neutrons between 0.8 and 18 MeV. In the data processing, a care was taken for the data correction for the effects of parasitic neutrons associated with primary neutrons; the correction proved to be of special importance in the present measurement. We compared the data obtained in the present experiment with the evaluated data, JENDL-3 and ENDF/B-IV (B-V for 12C), and discussed the origin of the discrepancies. The anisotropy observed for secondary neutrons from 238U and 232Th was found to be reproduced by Kalbach-Mann systematics on the assumption of isotropy of fission neutrons. The experimental results for 12C showed marked discrepancies concerning the scattering cross sections and neutron spectrum in the continuum region. (author)

  18. Non-destructive determination of 235U, 238U, 232Th and 40K concentrations in various consumed nuts and their implication on radiation dose levels to the human body

    International Nuclear Information System (INIS)

    The naturally occurring radionuclides of 238,235,234U,232Th and 40K and their daughter products are a potential source of radiation found in food. We have determined these five radiation sources in five popular consumed nuts. We used the following neutron activation analysis reactions of 238U(n,γ)239U, 232Th(n,γ)233Th and 41K(n,γ)42K to determine 238U and 232Th and 40K, respectively. Using known activity ratios of uranium stable isotopes we determined the activity of 234,235U, while 40K was found by the determined concentrations of 41K in the nuts. While the radiation doses are small we have established a reliable methodology to determine these radionuclides in typical edible nuts. (author)

  19. Standard practice for the determination of 237Np, 232Th, 235U and 238U in urine by inductively coupled plasma-Mass spectrometry (ICP-MS) and gamma ray spectrometry.

    CERN Document Server

    American Society for Testing and Materials. Philadelphia

    2005-01-01

    1.1 This practice covers the separation and preconcentration of neptunium-237 (237Np), thorium-232 (232Th), uranium-235 (235U) and uranium-238 (238U) from urine followed by quantitation using ICP-MS. 1.2 This practice can be used to support routine bioassay programs. The minimum detectable concentrations (MDC) for this method, taking the preconcentration factor into account, are approximately 1E-2Bq for 237Np (0.38ng), 2E-6Bq for 232Th (0.50ng), 4E-5Bq for 235U (0.50ng) and 6E-6Bq for 238U (0.48ng). 1.3 This standard does not purport to address all of the safety problems, if any, associated with its use. It is the responsibility of the user of this standard to establish appropriate safety and health practices and determine the applicability of regulatory limitations prior to use.

  20. Fiscal Year 2010 Phased Construction Completion Report for EU Z2-32 in Zone 2, East Tennessee Technology Park, Oak Ridge, Tennessee

    Energy Technology Data Exchange (ETDEWEB)

    Bechtel Jacobs

    2010-02-01

    The Record of Decision for Soil, Buried Waste, and Subsurface Structure Actions in Zone 2, East Tennessee Technology Park, Oak Ridge, Tennessee (DOEIORJO 1-2161 &D2) (Zone 2 ROD) acknowledged that most of the 800 acres in Zone 2 were contaminated, but that sufficient data to confirm the levels of contamination were lacking. The Zone 2 ROD further specified that a sampling strategy for filling the data gaps would be developed. The Remedial Design Report/Remedial Action Work Plan for Zone 2 Soils, Slabs, and Subsurface Structures, East Tennessee Technology Park, Oak Ridge, Tennessee (DOEIORIO 1 -2224&D3) (RDRJRAWP) defined the sampling strategy as the Dynamic Verification Strategy (DVS), generally following the approach used for characterization of the Zone I exposure units (EUs). The Zone 2 ROD divided the Zone 2 area into seven geographic areas and 44 EUs. To facilitate the data quality objectives (DQOs) of the DVS process, the RDR/RAWP regrouped the 44 EUs into 12 DQO scoping EU groups. These groups facilitated the DQO process by placing similar facilities and their support facilities together, which allowed identification of data gaps. The EU groups were no longer pertinent after DQO planning was completed and characterization was conducted as areas became accessible. As the opportunity to complete characterization became available, the planned DVS program was completed for the EU addressed in this document (EU Z2-32). The purpose of this Phased Construction Completion Report (PCCR) is to address the following: (1) Document DVS characterization results for EU Z2-32. (2) Describe and document the risk evaluation and determine if the EU meets the Zone 2 ROD requirements for unrestricted industrial use to 10 ft bgs. (3) Identify additional areas not defined in the Zone 2 ROD that require remediation based on the DVS evaluation results. (4) Describe the remedial action performed in the K-1066-G Yard in EU Z2-32. Approximately 18.4 acres are included in the EU

  1. Effects of the diacylglycerol o-acyltransferase 1 (DGAT1) K232A polymorphism on fatty acid, protein, and mineral composition of dairy cattle milk.

    Science.gov (United States)

    Bovenhuis, H; Visker, M H P W; Poulsen, N A; Sehested, J; van Valenberg, H J F; van Arendonk, J A M; Larsen, L B; Buitenhuis, A J

    2016-04-01

    Several studies have described associations between the diacylglycerol o-acyltransferase 1 (DGAT1) K232A polymorphism and routinely collected milk production traits but not much is known about effects of the DGAT1 polymorphism on detailed milk composition. The aim of this study was to estimate effects of the DGAT1 polymorphism on milk fatty acid, protein, and mineral composition. We looked for effects that were significant and consistent in Danish Holstein Friesian (HF), Danish Jersey, and Dutch HF as these are likely to be true effects of the DGAT1 K232A polymorphism rather than being effects of linked loci. For fatty acid composition, significant and consistent effects of the DGAT1 polymorphism were detected on C14:0, C16:0, C15:0, C16:1, C18:1 cis-9, conjugated linoleic acid (CLA) cis-9,trans-11, C18:2 cis-9,cis-12, and C18:3 cis-9,cis-12,cis-15 content (percent by weight, wt/wt %). For C16:0, C16:1, and C18:1 cis-9, the DGAT1 polymorphism explained more than 10% of the phenotypic variation. Significant effects on milk protein composition in Dutch HF could not be confirmed in Danish Jersey or Danish HF. For mineral content, significant and consistent effects of the DGAT1 polymorphism on calcium, phosphorus, and zinc were detected. In the Dutch HF population, the contribution of the DGAT1 K232A polymorphism to phenotypic variance was 12.0% for calcium, 8.3% for phosphorus, and 6.1% for zinc. Different from effects on fatty acid composition, effects of the DGAT1 polymorphism on yields of long-chain fatty acids C18:1 cis-9, CLA cis-9,trans-11, C18:2 cis-9,cis-12, and C18:3 cis-9,cis-12,cis-15 were not significant. This indicates that effects of DGAT1 on these fatty acids are indirect, not direct, effects: DGAT1 affects de novo synthesis of fatty acids and, consequently, the contribution of the long-chain fatty acids to total fat is decreased. In addition, effects of the DGAT1 polymorphism on yields of Ca, P, and Zn were not significant, which indicates that effects

  2. HI-resolution gamma spectrometry measurements of U-238, TH-232, K-40 and CS-137 concentrations in soil samples from Capao Island at CTEx

    Energy Technology Data Exchange (ETDEWEB)

    Oliveira, Luciano S.R.; Oliveira, Celio J.V.; Vilela, Paulo R.T.; Vital, Helio C., E-mail: vital@ctex.eb.br [Centro Tecnologico do Exercito (DDQBN/CTEX), Rio de Janeiro, RJ (Brazil). Div. de Defesa Quimica, Biologica e Nuclear. Secao de Defesa Nuclear

    2013-07-01

    Absolute soil concentrations of U-238, Th-232, K-40 and Cs-137 samples collected from Capao Island have been measured by using Hi-Resolution Gamma HPGe Spectrometry. The area of interest encompasses an embankment in a mangrove swamp in Guaratiba, Rio de Janeiro, where nuclear, chemical and biological defense laboratories of the Brazilian Army Technology Center (CTEx) are located. In order to ensure that no significant environmental impact has resulted from neutron physics experiments performed in a graphite subcritical assembly in addition to the operation of two cesium-driven irradiating facilities, routine monitoring of those isotopes have been regularly performed. A total of eight 250 ml samples of mangrove and embankment soils were extracted from four sites of known coordinates within an area of 300 x 300 m{sup 2} and remained stored for a minimum thirty-day period to allow equilibrium to be reached. Collection and preparation of samples were made according to previously established procedures. High purity germanium detectors were used to obtain high-resolution gamma spectra and counting times were required to exceed 30 hours in order to yield sufficient statistical accuracy. Energy and efficiency calibration curves of the counting system were determined by using the GENIE 2000 software for analysis of the gamma spectrum generated by nine standard sources with a total of 11 peak energies ranging from 0.05 to 1.3 MeV. The results, corrected for background, have been expressed as absolute specific activities. All experiments have been made in the Laboratory for Identification of Radiological Agents (LIAR) at CTEx. No trace of cesium-137 has been found and the measured levels of uranium-238, in the order of 10 Bq/kg, are close to the global mean. However, some data have been found to slightly exceed the expected normal range for thorium-232 (60% of samples) and potassium-40 (20% of samples). Since there is no handling of those isotopes in the site or others that

  3. Effects of the diacylglycerol o-acyltransferase 1 (DGAT1) K232A polymorphism on fatty acid, protein, and mineral composition of dairy cattle milk.

    Science.gov (United States)

    Bovenhuis, H; Visker, M H P W; Poulsen, N A; Sehested, J; van Valenberg, H J F; van Arendonk, J A M; Larsen, L B; Buitenhuis, A J

    2016-04-01

    Several studies have described associations between the diacylglycerol o-acyltransferase 1 (DGAT1) K232A polymorphism and routinely collected milk production traits but not much is known about effects of the DGAT1 polymorphism on detailed milk composition. The aim of this study was to estimate effects of the DGAT1 polymorphism on milk fatty acid, protein, and mineral composition. We looked for effects that were significant and consistent in Danish Holstein Friesian (HF), Danish Jersey, and Dutch HF as these are likely to be true effects of the DGAT1 K232A polymorphism rather than being effects of linked loci. For fatty acid composition, significant and consistent effects of the DGAT1 polymorphism were detected on C14:0, C16:0, C15:0, C16:1, C18:1 cis-9, conjugated linoleic acid (CLA) cis-9,trans-11, C18:2 cis-9,cis-12, and C18:3 cis-9,cis-12,cis-15 content (percent by weight, wt/wt %). For C16:0, C16:1, and C18:1 cis-9, the DGAT1 polymorphism explained more than 10% of the phenotypic variation. Significant effects on milk protein composition in Dutch HF could not be confirmed in Danish Jersey or Danish HF. For mineral content, significant and consistent effects of the DGAT1 polymorphism on calcium, phosphorus, and zinc were detected. In the Dutch HF population, the contribution of the DGAT1 K232A polymorphism to phenotypic variance was 12.0% for calcium, 8.3% for phosphorus, and 6.1% for zinc. Different from effects on fatty acid composition, effects of the DGAT1 polymorphism on yields of long-chain fatty acids C18:1 cis-9, CLA cis-9,trans-11, C18:2 cis-9,cis-12, and C18:3 cis-9,cis-12,cis-15 were not significant. This indicates that effects of DGAT1 on these fatty acids are indirect, not direct, effects: DGAT1 affects de novo synthesis of fatty acids and, consequently, the contribution of the long-chain fatty acids to total fat is decreased. In addition, effects of the DGAT1 polymorphism on yields of Ca, P, and Zn were not significant, which indicates that effects

  4. The influence of the nature of soil and plant and pollution on the 238U, 232Th, 222Rn and 220Rn concentrations in various natural honey samples using nuclear track detectors: Impact on the adult consumers

    Indian Academy of Sciences (India)

    M A Misdaq; A Mortassim

    2009-11-01

    238U and 232Th concentrations as well as 222Rn and 220Rn -activities per unit volume were measured in various natural honey samples collected from different regions in Morocco using CR-39 and LR-115 type II solid state nuclear track detectors (SSNTDs). These radionuclides were also measured in soils, plant flowers and nectar solutions corresponding to the honey samples studied. In addition, these radionuclides were measured in different imported honey samples. The measured 238U, 232Th, 222Rn and 220Rn concentrations ranged from (1.5 ± 0.1) mBq kg-1 to (10.6 ± 0.6) mBq kg-1, (1.1 ± 0.1) mBq kg-1 to (4.2 ± 0.2) mBq kg-1 , (1.5 ± 0.1) Bq kg-1 to (10.6 ± 0.6) Bq kg-1 and (1.1 ± 0.1) Bq kg-1 to (4.2 ± 0.2) Bq kg-1 for the honey samples studied, respectively. Annual 238U, 232Th and 222Rn intakes by Moroccan adults from the consumption of honey were assessed. The influence of the nature of soil and plant on the 238U and 232Th contents of the studied honey samples was investigated. These measurements were completed by an investigation of the 238U and 232 Th transfer between soils and plant flowers and that between plant flowers and honey, and also by the investigation of the influence of pollution due to different material dusts on 238U, 232Th and 222Rn in the honey samples studied. Committed equivalent doses due to the annual intake of 238U, 232Th and 222Rn were evaluated in the organs of adult members of the Moroccan rural population from the ingestion of the honey samples. The maximum total committed effective dose due to 238U, 232Th and 222Rn from the ingestion of natural honey by the Moroccan rural population was found to be equal to 0.64 Sv y-1 .

  5. Study of secondary neutron interactions with 232 Th, 129 I, and 127 I nuclei with the uranium assembly " QUINTA " at 2, 4, and 8 GeV deuteron beams of the JINR Nuclotron accelerator

    Energy Technology Data Exchange (ETDEWEB)

    Adam, J. [ASCR, Prague; Chilap, V. V. [IPTP, Dubna; Furman, M. G. [Dubna, JINR; Khushvaktov, J. [Dubna, JINR; Pronskikh, V. S. [Fermilab; Solnyshkin, A. A.. [Dubna, JINR; Stegailov, V. I. [Dubna, JINR; Suchopar, M. [ASCR, Prague; Tsoupko-Sitnikov, V. M. [Dubna, JINR; Tyutyunnikov, S. I. [Dubna, JINR; Vrzalova, J.. [Dubna, JINR; Wagner, V. [ASCR, Prague; Zavorka, L. [Dubna, JINR

    2016-06-01

    The natural uranium assembly, "QUINTA", was irradiated with 2, 4, and 8 GeV deuterons. The 232 Th, 127 I, and 129 I samples have been exposed to secondary neutrons produced in the assembly at a 20-cm radial distance from the deuteron beam axis. The spectra of gamma rays emitted by the activated 232 Th, 127 I, and 129 I samples have been analyzed and several tens of product nuclei have been identified. For each of those products, neutron-induced reaction rates have been determined. The transmutation power for the 129 I samples is estimated. Experimental results were compared to those calculated with well-known stochastic and deterministic codes.

  6. The proliferation potential of neptunium and americium

    Energy Technology Data Exchange (ETDEWEB)

    An, J. S.; Shin, J. S.; Kim, J. S.; Kwack, E. H.; Kim, B. K

    2000-05-01

    It is recognized that some trans-uranic elements other than plutonium, in particular Np and Am, if will be available in sufficient quantities, could be used for nuclear explosive devices. The spent fuel has been accumulating in number of nuclear power plant and operation of large scale commercial reprocessing plants. However, these materials are not covered by the definition of special fissionable material in the Agency Statute. At the time when the Statute was adopted, the availability of meaningful quantities of separated Np and Am was remote and they were not included in the definition of special fissionable material. Then, IAEA Board decided a measure for control of Np and Am on September 1999. This report contains the control method and the characteristic of Np and Am for using domestic nuclear industries, and it can be useful for understanding how to report and account of Np and Am. (author)

  7. Delocalization and new phase in Americium: theory

    Energy Technology Data Exchange (ETDEWEB)

    Soderlind, P

    1999-04-23

    Density-functional electronic structure calculations have been used to investigate the high pressure behavior of Am. At about 80 kbar (8 GPa) calculations reveal a monoclinic phase similar to the ground state structure of plutonium ({alpha}-Pu). The experimentally suggested {alpha}-U structure is found to be substantially higher in energy. The phase transition from fcc to the low symmetry structure is shown to originate from a drastic change in the nature of the electronic structure induced by the elevated pressure. A calculated volume collapse of about 25% is associated with the transition. For the low density phase, an orbital polarization correction to the local spin density (LSD) theory was applied. Gradient terms of the electron density were included in the calculation of the exchange/correlation energy and potential, according to the generalized gradient approximation (GGA). The results are consistent with a Mott transition; the 5f electrons are delocalized and bonding on the high density side of the transition and chemically inert and non-bonding (localized) on the other. Theory compares rather well with recent experimental data which implies that electron correlation effects are reasonably modeled in our orbital polarization scheme.

  8. Evaluation of neutron data for americium-241

    Energy Technology Data Exchange (ETDEWEB)

    Maslov, V.M.; Sukhovitskij, E.Sh.; Porodzinskij, Yu.V.; Klepatskij, A.B.; Morogovskij, G.B. [Radiation Physics and Chemistry Problems Inst., Minsk-Sosny (Belarus)

    1997-03-01

    The evaluation of neutron data for {sup 241}Am is made in the energy region from 10{sup -5} eV up to 20 MeV. The results of the evaluation are compiled in the ENDF/B-VI format. This work is performed under the Project Agreement CIS-03-95 with the International Science and Technology Center (Moscow). The Financing Party for the Project is Japan. The evaluation was requested by Y. Kikuchi (JAERI). (author). 60 refs.

  9. A four phases model to simulate the dispersion of 226Ra, 238U and 232Th in an estuary affected by phosphate rock processing

    International Nuclear Information System (INIS)

    A numerical model to simulate the dispersion of non conservative radionuclides in tidal waters has been developed. The model includes four phases: water, suspended matter and two grain size sediment fractions. Ionic exchanges between water and the solid phases have been formulated in terms of kinetic transfer coefficients instead of distribution coefficients, because the model was developed for nonequilibrium conditions. The model simultaneously solves the shallow water hydrodynamic equations, the suspended matter dispersion equation and the four equations which give the time evolution of specific activity in each phase. The model has been applied to the Odiel river (southwest Spain), where a phosphate complex releases its wastes. It gives good results in predicting concentrations of 226Ra, 238U and 232Th in water, suspended matter, distribution coefficients and Th/U mass rations. (author)

  10. Mass asymmetry dependence of fusion time-scales in 11B+237Np and 12C, 16O, 19F+232Th reactions in a dynamical trajectory model

    International Nuclear Information System (INIS)

    Dynamical trajectory calculations were carried out for the reactions of 11B+237Np and 12C, 16O and 19F+232Th, having mass asymmetries on either side of the Businaro-Gallone critical mass asymmetry αBG, in order to examine the mass asymmetry dependence of fusion reactions in these systems. The compound nucleus formation times were calculated as a function of the partial wave of the reaction for all the systems. This study brings out that for systems with αBG, the formation times are significantly larger than for α>αBG, which is caused by the dynamical effects involved in the large scale shape changes taking place in the fusion process as well as due to the interplay between the thermal and the collective motion during the collision process. The calculated time scales are comparable to the experimental values derived from the pre-fission neutron multiplicity measurements. (author). 16 refs., 4 figs., 1 tab

  11. Daily intakes of 238U, 234U, 232Th, 230Th, 228Th and 226Ra in the adult population of central Poland

    Energy Technology Data Exchange (ETDEWEB)

    Pietrzak-Flis, Z.; Rosiak, L.; Suplinska, M.M.; Chrzanowski, E.; Dembinska, S. [Central Laboratory for Radiological Protection, Konwaliowa 7, 03-194 Warsaw (Poland)

    2001-06-12

    Activity concentration of the uranium and thorium series radionuclides was determined in foodstuffs and drinking water in central Poland. Annual and daily intake for the adult population was estimated from the concentrations determined and average annual consumption of food and water. The daily intakes (in mBq) were 22.1 (238U), 26.5 (234U), 2.38 (232Th), 4.06 (230Th), 11.2 (228Th) and 42.2 (226Ra). The intake of uranium isotopes occurred mainly with water; the main intake of thorium isotopes was with animal products, vegetables, cereals and potatoes, whereas 226Ra entered mainly with animal products, cereals and vegetables. From the intake and dose coefficients, the annual effective doses for the ingested radionuclides were calculated. The annual effective dose was 5.95 {mu}Sv, of which 72.4% originated from 226Ra.

  12. Experimental Neutron-Induced Fission Fragment Mass Yields of 232Th and 238U at Energies from 10 to 33 MeV

    CERN Document Server

    Simutkin, V D; Blomgren, J; Österlund, M; Bevilacqua, R; Ryzhov, I V; Tutin, G A; Yavshits, S G; Vaishnene, L A; Onegin, M S; Meulders, J P; Prieels, R

    2013-01-01

    Development of nuclear energy applications requires data for neutron-induced reactions for actinides in a wide neutron energy range. Here we describe measurements of pre-neutron emission fission fragment mass yields of 232Th and 238U at incident neutron energies from 10 to 33 MeV. The measurements were done at the quasi-monoenergetic neutron beam of the Louvain-la-Neuve cyclotron facility CYCLONE; a multi-section twin Frisch-gridded ionization chamber was used to detect fission fragments. For the peak neutron energies at 33, 45 and 60 MeV, the details of the data analysis and the experimental results have been published before and in this work we present data analysis in the low-energy tail of the neutron energy spectra. The preliminary measurement results are compared with available experimental data and theoretical predictions.

  13. {sup 226}Ra, {sup 232}Th and {sup 40}K concentrations in igneous rocks from eastern desert, Egypt and its radiological implications

    Energy Technology Data Exchange (ETDEWEB)

    El-Arabi, A.M. [Physics Department, Faculty of Science Qena, South Valley University (Egypt)]. E-mail: elarabi21@yahoo.com

    2007-01-15

    By applying high-resolution {gamma}-ray spectroscopic system, the various radionuclides of the granite samples have been identified quantitatively based on the characteristic spectral peaks. The radionuclides {sup 226}Ra, {sup 232}Th and {sup 40}K concentrations measured as well as radiological parameters, for 49 granite samples were calculated. This subject is important in environmental radiological protection, since granites are widely used as building and ornamental stones. The variation in concentration of radionuclides for the Um Taghir area can be classified into two regions of low and high natural radioactivity. In old granite, the measured {gamma}-ray spectra, activity concentrations were determined for {sup 226}Ra (from 2.9+/-1 to 31.8+/-6Bqkg{sup -1}), {sup 232}Th (range from 1.4+/-1 to 14.9+/-4Bqkg{sup -1}) and {sup 40}K (from 132+/-11 to 2080+/-46Bqkg{sup -1}), in younger granite {sup 226}Ra (from 8.9+/-3 to 9087+/-95Bqkg{sup -1}), {sup 232}Th (range from 9.8+/-3 to 3834+/-62Bqkg{sup -1}) and {sup 40}K (from 471+/-22 to 10230+/-101Bqkg{sup -1}). In Wadi Karim area these values were (14.0+/-4-227.0+/-15, 10.5+/-3-183.0+/-14 and 2299+/-48-7356+/-86Bqkg{sup -1}). The highest values of {sup 226}Ra, {sup 232}Th and {sup 40}K concentration (9087+/-95, 3834+/-62 and 10230+/-101Bqkg{sup -1},respectively) were observed in anomalies samples at Um Taghir region. Radium-equivalent activities (Ra{sub eq}) in addition to the internal hazard index (H{sub in}) have also been determined. In Um Taghir samples Ra{sub eq} varies between 15 and 625Bqkg{sup -1} (old granite), 144-13982Bqkg{sup -1} (younger granite) which exceeds the permitted value (370Bqkg{sup -1}) and hazard index (H{sub in}) (0.05-1.74), (0.65-62.34) which is higher than 1, the corresponding values in Wadi Karim samples were 206-685Bqkg{sup -1} and from 0.59 to 2.46, respectively. The total absorbed dose rates in air calculated from the concentrations of the three radionuclides ranged from 8 to 6187n

  14. Neutron induced fission cross section ratios for 232Th, /sup 235,238/U, 237Np, and 239Pu from 1 to 400 MeV

    International Nuclear Information System (INIS)

    Time-of-flight measurements of neutron induced fission cross section ratios for 232Th, /sup 235,238/U, 237Np, and 239Pu, were performed using the WNR high intensity spallation neutron source located at Los Alamos National Laboratory. A multiple-plate gas ionization chamber located at a 20-m flight path was used to simultaneously measure the fission rate for all samples over the energy range from 1 to 400 MeV. Because the measurements were made with nearly identical neutron fluxes, we were able to cancel many systematic uncertainties present in previous measurements. This allows us to resolve discrepancies among different data sets. In addition, these are the first neutron-induced fission cross section values for most of the nuclei at energies above 30 MeV. 8 refs., 3 figs

  15. Search for quasifission in 12C + 238U and 18O + 232Th reactions at near and sub-barrier energies

    International Nuclear Information System (INIS)

    The main motivation of this present work is to study the onset of quasifission process in the fissility region > 0.8. It was observed that angular distribution of fission fragments produced in reaction in this fissility region showed anomalously large anisotropies at subbarrier energies as compared to SSPM, implying presence of pre-equilibrium fission. Here, mass-angle correlation studies of 12C + 238U and 18O + 232Th reactions has been reported, forming same compound nucleus 250Cf (Fissility = 0.86), at similar excitation energy and angular momentum. The measurements were carried out in the energy range Ecm /Vb ∼ 0.88 - 1.1, where Ecm is the energy in centre of mass frame and Vb is the Coulomb barrier

  16. Determination of environmental radioactivity (238U, 232Th and 40K) and indoor natural background radiation level in Chennai city (Tamilnadu State), India.

    Science.gov (United States)

    Babai, K S; Poongothai, S; Punniyakotti, J

    2013-01-01

    An extensive study on the determination of the natural radioactivity ((238)U, (232)Th and (40)K) levels in soil samples of Chennai city, India has been undertaken and the results of the same are compared with the levels reported in other Indian cities as well as other parts of the world. The radioactivity content in the soil samples, the absorbed dose rate, annual effective dose equivalent, radium equivalent activity, internal and external hazard indices were calculated and compared with UNSCEAR 2000 recommended values. In addition to the above, mapping of indoor natural background gamma radiation levels has been made using thermo luminescent dosemeters throughout Chennai city and the same are reported. PMID:22847868

  17. Motor' s Headlamp Testing Based on RS232 Serial Communications%基于串口通信的摩托车前照灯检测

    Institute of Scientific and Technical Information of China (English)

    王晓丽

    2009-01-01

    针对传统的摩托车灯光检测硬件电路复杂和易受干扰的不足,提出了一种新型的基于串口通信的摩托车灯光测试方法.将工控机和灯光仪利用串口线相连,在VC++6.0环境下利用MSComm控件编写RS232串口通信程序,实现了工控机对灯光仪数据的采集、数据显示和结果判断.实际运行结果表明,该方法硬件电路简单、成本低和传输数据不易受干扰.

  18. Distribution of Natural (U-238, Th-232, Ra-226) and Technogenic (Sr-90, Cs-137) Radionuclides in Soil-Plants Complex Near Issyk-Kul Lake, Kyrgyzstan

    Science.gov (United States)

    Jovanovic, L.; Kaldybaev, B.; Djenbaev, B.; Tilenbaev, A.

    2012-04-01

    Researches on radionuclides distribution in the soil-plants complex provide essential information in understanding human exposure to natural and technogenic sources of radiation. It is necessary in establishing regulation relating to radiation protection. The aim of this study was the radiochemical analysis of the content natural radionuclides 238U, 232Th,226Ra and technogenic radionuclides content (90Sr, 137Cs) in soils near Issyk-Kul lake (Kyrgyzstan). Results of radiochemical analyses have shown, that the concentrations of thorium-232 are fluctuating in the limits (11.7-84.1)-10-4% in the soils. The greatest concentration of thorium-232 has been found in the light chestnut soils. The content of uranium-238 in the soils near Issyk-Kul lake is fluctuating from 2.8 up to 12.7-10-4%. Radium-226 has more migration ability in comparison with other heavy natural radionuclides. According to our research the concentrations of radium-226 are fluctuating in the limits (9.4-43.0)-10-11%. The greatest concentration of radium-226 (43,0±2,8)-10-11% has been determined in the light chestnut soil. In connection with global migration of contaminating substances, including radioactive, the special attention is given long-lived radionuclides strontium-90 and caesium-137 in food-chains, and agroecosystems. Results of radiochemical analyses have shown, that specific activity of strontium-90 is fluctuating in the range of 2.9 up to 11.1 Bq/kg, and caesium-137 from 3.7 up to 14,3 Bq/kg in the soil of agroecosystems in the region of Issyk-Kul. In soil samples down to 1 meter we have observed vertical migration of these radionuclides, they were found to accumulate on the surface of soil horizon (0-5 cm) and their specific activity sharply decreases with depth. In addition in high-mountain pastures characterized by horizontal migration of cattle in profiles of soil, it was discovered that specific activity of radionuclides are lower on the slope than at the foot of the mountain. The

  19. The dietary intake of 238U, 234U, 230Th, 232Th, 228Th and 226Ra from food and drinking water by inhabitants of the Walbrzych region

    International Nuclear Information System (INIS)

    Intake with food and water of the natural radionuclides of the uranium and thorium series was determined for adult population of the south-western region in Poland, where in the 1950-ies an exploration of uranium ore was conducted. Concentration of the radionuclides was determined in food products and drinking water and their annual intake was estimated on the basis of the average annual consumption. The intake of 238U, 234U and 230Th occurred mainly with water (33% to 68%), whereas the intake of 232Th, 228Th and 226Ra was mainly with vegetables, potatoes, milk and flour. From the intake and dose coefficients the annual effective doses from the ingested radionuclides were calculated. The total dose was 5.6μSv, of which 74% originated from 226Ra. (author)

  20. Daily intakes of 238U, 234U, 232Th, 230Th, 228Th and 226Ra in the adult population of central Poland

    International Nuclear Information System (INIS)

    Activity concentration of the uranium and thorium series radionuclides was determined in foodstuffs and drinking water in central Poland. Annual and daily intake for the adult population was estimated from the concentrations determined and average annual consumption of food and water. The daily intakes (in mBq) were 22.1 (238U), 26.5 (234U), 2.38 (232Th), 4.06 (230Th), 11.2 (228Th) and 42.2 (226Ra). The intake of uranium isotopes occurred mainly with water; the main intake of thorium isotopes was with animal products, vegetables, cereals and potatoes, whereas 226Ra entered mainly with animal products, cereals and vegetables. From the intake and dose coefficients, the annual effective doses for the ingested radionuclides were calculated. The annual effective dose was 5.95 μSv, of which 72.4% originated from 226Ra

  1. Spectroscopy study after quasi-elastic collision in the system 208Pb+232Th at an incident energy of 17 MeV per nucleon

    International Nuclear Information System (INIS)

    In the present thesis by means of a particle-particle-γ and particle-particle-neutron coincidence experiment γ and neutron spectroscopic studies after quasi-elastic collisions at incident energies far above the Coulomb barrier were performed. For the study of the γ decay by the necessary correction of the Doppler shift the possibility results to study excitations in the projectile and in the target. So in the case of 232Th beside the observation of the ground state band up to the spin 14 ℎ also a very large number of transitions from vibrational side bands. From the spectra the γ emission probabilities in dependence on the distance of closest approximation were extracted. (orig./HSI)

  2. The learning of the evolution and temporary characteristics of the decay nuclei 14C, 238U, 232Th, 40K, 87Rb

    International Nuclear Information System (INIS)

    Quantum-mechanical method, which was proposing earlier for the theoretical description of the resonance scattering of the γ-quantum, was generalizing with Doppler effect using. New algorithm for the definition of the characteristic functions for the energy distribution, decay probability and decay functions elaborated. It gives possibility more precise estimate temporary characteristics of the nuclei chronometers and to define a number of the steps of the γ-absorption γ-emission in the decay process. It is give the quantum- mechanical ground of the necessity of revision of the temporary characteristics of the nuclei-chronometers. The calculations have been doing for the concrete case decay of exited nuclei 14C, 238U, 232Th, 40K, 87Rb under room temperature taking into account Doppler effect and without it. 4 refs., 1 tab., 6 figs

  3. Delayed neutron and delayed photon characteristics from photofission of 232Th, 235,238U, and 237Np with endpoint Bremsstrahlung photons in the giant dipole resonance region

    Science.gov (United States)

    Doré, D.; Dighe, P. M.; Berthoumieux, E.; Laborie, J.-M.; Ledoux, X.; Macary, V.; Panebianco, S.; Ridikas, D.

    2009-10-01

    A renewed interest in photonuclear reactions was stimulated by applications as radioactive ion beam production, irradiation stations by high energy photons, shielding of electron accelerators, etc. Today, a particular attention is paid to the non-destructive characterization of waste barrels and the detection of nuclear materials, both based on photofission process and the associated delayed neutron (DN) and delayed photon (DP) emissions. The need of accurate and complete data for DN and DP yields and time characteristics of actinides was the motivation for an experimental campaign, started in 2004. In this paper, the experimental setup and the data analysis method will be presented and the modeling work will be described. Experimental results for DN and DP characteristics will be compared to calculations in the case of photofission of 232Th, 235,238U, and 237Np.

  4. Assessment of radiological impact in mineral industrial plants caused by deposition of wastes with U{sup 238} and/or Th{sup 232} associated

    Energy Technology Data Exchange (ETDEWEB)

    Ladeira, Paula C.; Alves, Rex Nazare, E-mail: rexnazare@ime.eb.b [Instituto Militar de Engenharia (IME), Rio de Janeiro, RJ (Brazil); Ruperti Junior, Nerbe J., E-mail: nruperti@cnen.gov.b [Comissao Nacional de Energia Nuclear (DIREJ/CNEN-RJ), Rio de Janeiro, RJ (Brazil). Div. de Rejeitos Radioativos

    2011-07-01

    The industrial-mining facilities constantly produce, in Brazil and in abroad, wastes from its production, many times containing uranium and/or thorium associated. Due to the large quantities generated, these wastes are usually deposited at the site of the facility, close to the place where they were produced. Since the chains of radioactive U{sup 238} and Th{sup 232} with alpha-emitting radionuclides have long half-life, waste deposits associated with these elements may cause radiological impact on the man and on the environment, even in the long term. Mathematical models are often used to represent the biosphere and the transport of radionuclides near to the surface. Thus, it was decided, through the software {sup M}athematica{sup ,} to present a methodology based on the solution of Bateman equations for the calculation of radiological impact on individuals from the public exposed to contamination. The radiological impact appraisal was carried out considering a scenario of intrusion into landfills containing U{sup 238} and / or Th{sup 232} in post-operational phase of an industrial-mining installation. The critical group examined was represented by farmers who used water from an artesian well for daily consumption and which feed themselves on vegetables locally grown in clay soil. As a result, there was the exposure in pathways evaluated, a minor contribution of dose for ingestion of contaminated water. The conclusion of this work, show us that calculated doses were within the accepted international limits for the intrusion scenario. Parameters associated with mathematical models defining the choice of project to build a landfill for the purpose of deposition, whereas rates of doses can be estimated in each of the scenarios proposed. (author)

  5. Identifikasi Secara Serologi Galur Virus Flu Burung Subtipe H5N1 Clade 2.1.3 dan Clade 2.3.2 pada Ayam Petelur (SEROLOGICAL IDENTIFICATION OF AVIAN INFLUENZA STRAIN VIRUS SUBTYPE H5N1 CLADE 2.1.3 AND CLADE 2.3.2 FROM LAYER

    Directory of Open Access Journals (Sweden)

    Aprilia Kusumastuti

    2015-10-01

    Full Text Available The aim of the study was to know avian influenza (AI infection in field by using serology test in threemarketing area of AI vaccines. Haemagglutination inhibition methode was used in this test. There werefour antigen strains of AI subtype H5N1 clade 2.1.3 (AIstrainA/Chicken/West Java/PWT-WIJ/2006, AIstrain A/Chicken/Garut/BBVW-223/2007, AI strain A/Chicken/West Java-Nagrak/30/2007, and AI strainA/Chicken/Pekalongan/BBVW-208/2007 and 2 antigen strains of AI subtype H5N1 clade 2.3.2 (AI strainA/duck/Sukoharjo/BBVW-1428-9/2012 and AI strain A/duck/Sleman/BBVW-1463-10/2012 was used inthis study for HI test. The result presents that 93,33% chicken farms in three marketing area of PT. SanbioLaboratories have positive antibody titre to AI subtype H5N1 clade 2.1.3. This titre may be obtained fromAI clade 2.1.3 vaccination. From 15 samples, 92,86% are positive to AI subtype H5N1 clade 2.3.2A/duck/Sukoharjo/BBVW-1428-9/2012 and 92,31% are positive to A/duck/Sleman/BBVW-1463-10/2012 evenwithout AI clade 2.3.2 vaccination. This antibody titre may be obtained from AI clade 2.1.3 vaccine crossprotection or field infection.

  6. A novel del(8)(q23.2q24.11) contributing to disease progression in a case of JAK2/TET2 double mutated chronic myelomonocytic leukemia

    DEFF Research Database (Denmark)

    Toft-Petersen, Marie; Kjeldsen, Eigil; Nederby, Line;

    2014-01-01

    relevant for leukemogenesis. While a frameshift mutation in the TET2 gene was stably present throughout the course of disease the JAK2 mutation was acquired after initial diagnosis of CMML. At progression aCGH revealed del(8q)(q23.2q24.11) encompassing various cancer relevant genes of which RAD21 and CSMD3...

  7. Transfer Rates of 238U and 232Th for E. globulus, A. mearnsii, H. filipendula and Hazardous Effects of the Usage of Medicinal Plants From Around Gold Mine Dump Environs

    Directory of Open Access Journals (Sweden)

    Victor M. Tshivhase

    2015-12-01

    Full Text Available Medicinal plant consumption can be a source of human exposure to radioactive elements such as 238U and 232Th, which can lead to internal radiation doses. The uptake of 238U and 232Th from soils to the leaf samples of three different medicinal plant species (Eucalyptus globulus, Acacia mearnsii and Hyparrhenia filipendula from the purlieu of the Princess gold mine dump, an abandoned contaminated tailings storage site (TSS, located at longitude 27°55′00″E and latitude 26°09′30″S in Davidsonville (Roodepoort, west of Johannesburg, South Africa was measured. This was done using ICP-MS spectrometry and substantial differences were observed in the soil-plant transfer factor (TF values between these radionuclides. The plant species E. globulus exhibited the highest uptake of 238U, with an average TF of 3.97, while that of H. filipendula was 0.01 and the lowest TF of 0.15 × 10−2 was measured for A. mearnsii. However, in the case of 232Th, the highest average TF was observed for A. mearnsii (0.29, followed by E. globulus (0.10 and lowest was measured for H. filipendula (0.27 × 10−2. The ratio of TF average value i.e., 238U to 232Th in the soil-plant leaves was 38.05 for E. globulus, 0.01 for A. mearnsii and 4.38 for H. filipendula.

  8. Assignment of FUT8 to chicken chromosome band 5q1.4 and to human chromosome 14q23.2-->q24.1 by in situ hybridization. Conserved and compared synteny between human and chicken

    NARCIS (Netherlands)

    Coullin, Ph.; Crooijmans, R.P.M.A.; Groenen, M.A.M.; Heilig, R.; Mollicone, R.; Oriol, R.; Candelier, J.J.

    2002-01-01

    The human FUT8 gene is implicated in crucial developmental stages and is overexpressed in some tumors and other malignant diseases. Based on three different experiments we have assigned the FUT8 gene to chromosome bands 14q23.2 --> q24.1 and not 14q24.3 as previously shown (Yamaguchi et al., 1999

  9. 2-[3-(2-取代苯基)-1H-吡唑-1-基]-4,6-二甲氧基嘧啶类化合物的合成及除草活性研究%Synthesis and Herbicidal Activities of 2-[3-(2-Substitutedphenyl)- 1H-pyrazol-yl]-4,6-dimethoxypyrimidine Derivatives

    Institute of Scientific and Technical Information of China (English)

    李元祥; 林龙; 陈琼

    2011-01-01

    Twenty two novel 2-[3-(2-substitutedphenyl)-1H-pyrazol-1-yl]-4,6-dimethoxypyrimidine derivatives have been designed and synthesized using 1-(2-hydroxyphenyl)ethanone as starting material.All synthesized compounds were confirmed by 1H NMR, MS techniques and elemental analysis.The preliminary bioassay showed that some of them exhibited certain herbicidal activities.%以邻羟基苯乙酮为起始原料,设计合成了22个新型的2-[3-(2-取代苯基)-1H-吡唑-1-基]-4,6-二甲氧基嘧啶类化合物,通过1H NMR,MS和元素分析对所合成的化合物进行了结构表征.初步生物活性测试结果表明.在试验浓度下部分化合物具有一定的除草活性.

  10. Use of LabSOCS for determination of specific concentrations of {sup 40}K, {sup 238}U and {sup 232}Th in fertilizer samples; Uso de LabSOCS no calculo da eficiencia de detecao para determinacao da concentracao especifica de {sup 40}K, {sup 238}U e {sup 232}Th em amostras de fertilizantes

    Energy Technology Data Exchange (ETDEWEB)

    Garcez, Ricardo Washington Dutra; Lopes, Jose Marques; Silva, Ademir Xavier da, E-mail: rgarcez@con.ufrj.br, E-mail: marqueslopez@yahoo.com.br [Coordenacao dos Programas de Pos-Graduacao em Engenharia (COPPE/UFRJ), Rio de Janeiro, RJ (Brazil). Programa de Engenharia Nuclear; Domingues, Alessandro Mariano; Lima, Marco Frota, E-mail: slessandrodomingues@fisica.if.uff.br, E-mail: marcofrotalima@yahoo.com.br [Universidade Federal Fluminense (UFF), Niteroi, RJ (Brazil). Instituto de Biologia

    2015-07-01

    Use of fertilizer is an established practice worldwide to promote agricultural productivity increased without increasing the planted area, resulting in native forests protection and increase of the food availability. Some kinds of fertilizer have in their chemical composition some radionuclides due the origin of its feedstock, such as {sup 238}U, the {sup 232}Th, and their descendants, beyond {sup 40}K. Knowledge of the radioactivity levels in the environment is great importance to know the gamma radiation dose that the human being is exposed. For identification and quantitation of radionuclides, it was used gamma spectrometry where HPGe detector was used to obtain the spectra, and LabSOCS software for calculating the detection efficiency for each energy. The values of {sup 232}Th specific concentrations ranged from 4.1 to 368.1 Bq.Kg{sup -1} , the values of {sup 238}U specific concentrations ranged from 16.0 to 647.7 Bq.Kg{sup -1} and {sup 40}K specific concentrations ranged from 19.1 to 12713 Bq.Kg{sup -1} . Concentrations of values are consistent with those found in literature. (author)

  11. Assessment of sedimentation rate based on disequilibrium in the {sup 232}Th decay series in an artificial pond downstream a former uranium mine

    Energy Technology Data Exchange (ETDEWEB)

    Reyss, J.L. [Laboratoire des Sciences du Climat et de l' Environnement - LSCE/IPSL, Unite Mixte de Recherche 8212 CEA, CNRS, UVSQ, F-91198 Gif-sur-Yvette Cedex (France); Mangeret, A.; Courbet, C.; Saadi, Z.; Guillevic, J. [Institut de Radioprotection et de Surete Nucleaire (IRSN), BP 17, 92262 Fontenay aux Roses (France); Thouvenot, A. [LMGE, UMR CNRS 6023, Lab Microorganismes Genome et Environnement, 63 177 Aubiere (France)

    2014-07-01

    In rivers and lakes, sediment dynamics are very difficult to quantify by field measurements as well as by modeling studies (Olley et al. 1997 WRR 33, 1319-1326). The well-known {sup 210}Pb excess method (Appleby 2000 Limnology 59-S.1, 1-14; Perga et al. 2010 Limnol. and Ocean. 55, 803-816) cannot be used for quantifying sedimentation rates over granitic catchments as large amounts of {sup 210}Pb produced by granite weathering tend to dilute the atmospheric {sup 210}Pb. The knowledge of sedimentation rates in lakes is however very important for understanding the geochemical mechanisms involved in contaminant scavenging and remobilization at the sediment-water interface (SWI). Moreover, these measurements are crucial for developing solute transport models, especially for radionuclides and metals in pore waters and through the SWI. In order to overcome these issues, this study focuses on an artificial pound located in a granitic catchment, down-gradient from a former uranium mining site that ceased operations at the beginning of the 80's (Guillevic and Reyss 2011 ICRER 2011). Sediment sampling was carried out in this artificial lake with an UWITEC{sup R} hand corer. All the samples were dried and the activities of artificial and natural radionuclides were measured by gamma spectrometry, at the Underground Laboratory of Modane and alpha spectrometry after radiochemical purification. The profile of {sup 210}Pb activities in the sediment increased with depth in the core and did not allow to distinguish the atmospheric {sup 210}Pb from the {sup 210}Pb produced by watering processes in this uranium enriched environment. Another method for quantifying sediment accumulation rates is therefore proposed here using the disequilibrium between {sup 228}Ra (half-life of 5.75 years) and {sup 232}Th, the parent isotope. The excess of {sup 228}Ra over its respective parent {sup 232}Th has already been demonstrated by (Olley et al. 1997 WRR 33, 1319-1326) in river and lake

  12. 238U series isotopes and 232Th in carbonates and black shales from the Lesser Himalaya: implications to dissolved uranium abundances in Ganga-Indus source waters.

    Science.gov (United States)

    Singh, S K; Dalai, Tarun K; Krishnaswami, S

    2003-01-01

    238U and (232)Th concentrations and the extent of (238)U-(234)U-(230)Th radioactive equilibrium have been measured in a suite of Precambrian carbonates and black shales from the Lesser Himalaya. These measurements were made to determine their abundances in these deposits, their contributions to dissolved uranium budget of the headwaters of the Ganga and the Indus in the Himalaya and to assess the impact of weathering on (238)U-(234)U-(230)Th radioactive equilibrium in them. (238)U concentrations in Precambrian carbonates range from 0.06 to 2.07 microg g(-1). The 'mean' U/Ca in these carbonates is 2.9 ng U mg(-1) Ca. This ratio, coupled with the assumption that all Ca in the Ganga-Indus headwaters is of carbonate origin and that U and Ca behave conservatively in rivers after their release from carbonates, provides an upper limit on the U contribution from these carbonates, to be a few percent of dissolved uranium in rivers. There are, however, a few streams with low uranium concentrations, for which the carbonate contribution could be much higher. These results suggest that Precambrian carbonates make only minor contributions to the uranium budget of the Ganga-Indus headwaters in the Himalaya on a basin wide scale, however, they could be important for particular streams. Similar estimates of silicate contribution to uranium budget of these rivers using U/Na in silicates and Na* (Na corrected for cyclic and halite contributions) in river waters show that silicates can contribute significantly (approximately 40% on average) to their U balance. If, however, much of the uranium in these silicates is associated with weathering resistant minerals, then the estimated silicate uranium component would be upper limits. Uranium concentration in black shales averages about 37 microg g(-1). Based on this concentration, supply of U from at least approximately 50 mg of black shales per liter of river water is needed to balance the average river water U concentration, 1.7 microg L

  13. Assessment of natural radionuclides concentration from 238U and 232Th series in Virginia and Burley varieties of Nicotiana tabacum L

    International Nuclear Information System (INIS)

    Brazil is the largest exporter and second largest producer of tobacco worldwide, according to the crop production of 2013/2014. The tobacco plant (Nicotiana tabacum L.) is used to manufacture all derivatives and the chemical composition of the resulting tobacco products varies with the type of tobacco leaves, how they are grown, the region where they are cultivated, the characteristics of preparation (compression, filter and paper) and the temperature variations resulting from the incomplete combustion of tobacco. Tobacco products are extensively used throughout the world, and the most consumed are cigarettes, cigars and narghile. The damaging effects that these products cause to human health are discussed globally, and many surveys are performed with the aim of relating the use of these products with various illnesses. There is a lack of information about the radiological characterization of the tobacco plant both in international and Brazilian literature. The objective of this study was to determine the concentration of radionuclides 238U, 234U, 230Th, 22'6Ra, 210Pb and 210Po, members from the 238U decay series, and the radionuclides 232Th and 228Ra members of the 232Th decay series in the varieties Burley and Virginia, which are the most cultivated in Brazil. Plants from these varieties were cultivated in pots with organic substrate and fertilizer and also acquired from the producers and analyzed by alpha spectrometry for U and Th isotopes and 210Po determination, and gross alpha and beta counting, 228Ra, 226Ra and 210Pb determination. The whole plant, from both places, was analyzed; root, stem, leaves, as well as the organic substrate, the fertilizers, and the soil. The results for U and Th isotopes presented values below the detection limits of the methods to the leaves and stems of all plants analyzed, with measurable results only in roots, soil, and substrate. The radionuclides 226Ra, 228Ra, 210Pb, and 210Po, were determined in most parts of the plants

  14. Analyzing urine ketone of 235 medical examiners%232例体检者尿酮体阳性结果分析

    Institute of Scientific and Technical Information of China (English)

    王会敏; 何柯新

    2012-01-01

    目的 探讨尿酮体在体检人群不同年龄段、不同性别的分布及其与血糖的相关性.方法 对232例尿酮体为阳性的体检者按年龄及性别分组进行分析,同时与其同期检测的血糖结果 进行对比分析.结果 尿酮体阳性者以1+和2+为主;主要出现在20~50岁年龄段中;大多数尿酮体阳性者其血糖不高(≤6.1).结论 在体检人群中尿酮体阳性与血糖高低不存在相关性,尿酮体阳性并不能准确反映患者的血糖水平;尿酮体阳性主要集中在20~50岁年龄组.%Objective Objective: To explore the relationship between urine ketone and different age and gender and plasma glucose detected in the same time with urine ketone. Methods The results of totally 232 medical examiners whose urine ketone were positive were analyzed according to different ages and genders. Results The urine ketone results which are positive are 1+ and 2 + , mainly distribute the ages of 20 to 50. And great majority of them has a normal or low level of fasting plasma glucose. Conclusion The urine ketone which are positive has no relationship with plasma glucose,it can't accurately reflect the level of plasma glucose. We found that most of the groups distribute the ages of 20 to 50. The reasons probably are they have heavy work pressure and imbalanced diet. People need to pay attention to the quality of life. Having a balanced nutrition diet and eating on time will be a good life style.

  15. Determination of natural radionuclides from 238U and 232Th series, trace and major elements in sediment cores from baixada Santista and evaluation of impacted areas

    International Nuclear Information System (INIS)

    Baixada Santista is the region of higher population of the coast of Sao Paulo State, where it is located the largest port in Latin America, in the city of Santos, and the most important industrial complex of Latin America, in the city of Cubatao. This region has received in recent years a considerable load of industrial and domestic effluents in its water bodies, as a direct result of the industrial and port activities and the large population growth in recent decades, and is considered nowadays highly impacted. In the present study sediment cores were collected in the estuary of Santos-Cubatao, in the estuary of Sao Vicente, in the channel of Bertioga and Santos Bay, in order to determine the concentration of trace and major elements and natural radionuclides from the 238U and 232Th series. The techniques used were neutron activation analysis, X-ray fluorescence and gamma spectrometry, respectively. The obtained values for the elements Cr, Sb, Ta and Zn in some cores, are higher than data from literature, and can indicate a possible anthropic contribution. Comparing the obtained values of Cr and Zn elements determined in the sediment cores with the values of TEL and PEL index for sediment quality, it was verified that the studied region presents Cr levels higher than TEL in Santos-Cubatao estuary and Bertioga channel and Zn element presented values higher than TEL for some core slices of Santos-Cubatao estuary, for one core of Sao Vicente estuary, one core in Bertioga channel and Santos Bay. For the other elements, the values obtained in this study can be considered as reference values for the region. Although the element As presented higher values than the TEL in all the studied environments, the concentrations obtained are of the same order of magnitude as literature data and, therefore, can be considered also as reference values for the region. No enrichment was found for the major elements in all the ecosystems studied, with the exception for the element P

  16. Measurement of the fission cross section induced by fast neutrons of the {sup 232}Th/{sup 233}U nuclei within the innovating fuel cycles framework; Mesure de la section efficace de fission induite par neutrons rapides des noyaux {sup 232}Th/{sup 233}U dans le cadre des cycles de combustible innovants

    Energy Technology Data Exchange (ETDEWEB)

    Grosjean, C

    2005-03-15

    The thorium-U{sup 233} fuel cycle might provided safer and cleaner nuclear energy than the present Uranium/Pu fuelled reactors. Over the last 10 years, a vast campaign of measurements has been initiated to bring the precision of neutron data for the key nuclei (Th{sup 232}, Pa{sup 233} and U{sup 233}) at the level of those for the U-Pu cycle. This is the framework of these measurements, the energy dependent neutron induced fission cross section of Th{sup 232} and U{sup 233} has been measured from 1 to 7 MeV with a target accuracy lesser than 5 per cent. These measurements imply the accurate determination of the fission rate, the number of the target nuclei as well as the incident neutron flux impinging on the target, the latter has been obtained using the elastic scattering (n,p). The cross section of which is very well known in a large neutron energy domain ({approx} 0,5 % from 1 eV to 50 MeV) compared to the U{sup 235}(n,f) reaction. This technique has been applied for the first time to the Th{sup 232}(n,f) and U{sup 233}(n,f) cases. A Hauser-Feshbach statistical model has been developed. It consists of describing the different decay channels of the compound nucleus U{sup 234} from 0,01 to 10 MeV neutron energy. The parameters of this model were adjusted in order to reproduce the measured fission cross section of U{sup 233}. From these parameters, the cross sections from the following reactions could be extracted: inelastic scattering U{sup 233}(n,n'), radiative capture U{sup 233}(n,{gamma}) and U{sup 233}(n,2n). These cross sections are still difficult to measure by direct neutron reactions. The calculated values have allowed us to fill the lack of experimental data for the major fissile nucleus of the thorium cycle. (author)

  17. Synthesis, Spectral and Electrochemical Properties and DFT Studies of Two Complexes of Ruthenium with Bis-2,3-(2-PyridylPyrazine and 4-Picoline

    Directory of Open Access Journals (Sweden)

    Chhandasi Guharoy Sarkar

    2016-06-01

    Full Text Available Reaction of bis-2,3-(2-pyridylpyrazine (L with [Ru(dmso4Cl2] in presence of 4-picoline (L1 affords mixed- ligand complexes of the type [Ru2L(L14Cl4] in which ligand, L binds to the metal center in the bridging, bidentate N,N fashion forming two five-membered chelate rings. Along with [Ru2L(L14Cl4], another complex of the type [Ru(L12(dmso2Cl2] is formed. All the complexes are diamagnetic, and show characteristic 1H NMR signals and intense MLCT transitions in the visible region. DFT studies reveal that the HOMO of the complexes is mostly based on the metal center while the LUMO has maximum contribution from the bonded 4-picoline ligand. Cyclic voltammetry on these complexes shows a Ru(II-Ru(III oxidation on the positive side of SCE followed by a reduction of the coordinated 4-picoline ligand on the negative side of SCE.

  18. {sup 230}Th, {sup 232}Th and {sup 238}U determinations in phosphoric acid fertilizer and process products by ICP-MS

    Energy Technology Data Exchange (ETDEWEB)

    Nascimento, Marcos R.L. do; Guerreiro, Luisa M.R.; Bonifacio, Rodrigo L.; Taddei, Maria H.T., E-mail: pmarcos@cnen.gov.br [Comissao Nacional de Energia Nuclear (LAPOC/CNEN-MG), Pocos de Caldas, MG (Brazil). Laboratorio de Pocos de Caldas

    2015-07-01

    Through processing of Santa Quiteria-CE mine phosphate rock, Brazil has established a project for production of phosphoric acid fertilizer and uranium as a by-product. Under leaching conditions of phosphate rock with sulfuric acid, which is the common route for preparing phosphoric acid fertilizer, a large part of uranium, thorium and their decay products naturally present in the rock are solubilized. In order to assess the contamination potential in phosphoric acid and others process products, this paper describes a previous precipitation and direct methods for routine analysis of thorium and uranium isotopes by ICP-MS. In all samples, {sup 230}Th, {sup 232}Th and {sup 238}U were directly determined after dilution, except {sup 230}Th in phosphoric acid loaded with uranium sample, which to overcome equipment contamination effect, was determined after its separation by oxalate precipitation using lanthanum as a carrier. The results obtained by the proposed method by ICP-MS, were in good agreement when compared to alpha spectrometry for {sup 230}Th, and ICP-OES and spectrophotometry with arsenazo III for elementary uranium and thorium determinations. (author)

  19. Vertical and horizontal distribution of radionuclides (232Th, 238U and 40K) in sediment from Manjung coastal water area Perak, Malaysia

    Science.gov (United States)

    Abdullah, Anisa; Hamzah, Zaini; Saat, Ahmad; Wood, Ab. Khalik

    2016-01-01

    Distribution of radionuclides from anthropogenic activities has been widely studied in marine coastal area. Due to rapid population growth and socio-economic development in Manjung area such as coal fired power plant, iron foundries, port development, waste discharged from factories and agriculture runoff may contribute to increase in pollution rate. The radioactive materials from anthropogenic activities could deteriorate the quality of the marine ecosystem and thus lead to possible radiological health risk to the population. Radionuclides (232Th, 238U and 40K) content in surface and profile sediment from Manjung coastal area was determined in this study. Radionuclides in sediment from seven locations were collected using sediment core sampling and measurements were carried out using Energy Dispersive X-ray Fluorescence (EDXRF) spectroscopy. The results show that the concentration of radionuclides in surface sediment and distribution trend of depth vertical profile sediment generally varies depending on locations. Enrichment factors (EF), geo-accumulation index (Igeo) and pollution index (PI) were applied to determine level of pollution of this study area. The radiological risks related to human exposure were evaluated based on external hazard index (Hex).

  20. Capture and Fission rate of 232-Th, 238-U, 237-Np and 239-Pu from spallation neutrons in a huge block of lead.

    CERN Document Server

    Vlachoudis, Vasilis

    2000-01-01

    The study is centered on the research of the incineration possibility of nuclear waste, by the association of a particle accelerator with a multiplying medium of neutrons, in the project "Energy Amplifier" of C. Rubbia. It consists of the experimental determination of the rates of capture and fission of certain elements (232-Th, 238-U, 237-Np and 239-Pu) subjected to a fluence of fast spallation neutrons. These neutrons are produced by the interaction of high kinetic energy protons (several GeV) provided by the CERN-PS accelerator, on a large lead solid volume. The measurement techniques used in this work, are based on the activation of elements in the lead volume and the subsequent gamma spectroscopy of the activated elements, and also by the detection of fission fragment traces. The development, of a Monte Carlo code makes it possible, on one hand, to better understand the relevant processes, and on the other hand, to validate the code, by comparison with measurements, for the design and the construction of...

  1. Disease-related growth factor and embryonic signaling pathways modulate an enhancer of TCF21 expression at the 6q23.2 coronary heart disease locus.

    Directory of Open Access Journals (Sweden)

    Clint L Miller

    Full Text Available Coronary heart disease (CHD is the leading cause of mortality in both developed and developing countries worldwide. Genome-wide association studies (GWAS have now identified 46 independent susceptibility loci for CHD, however, the biological and disease-relevant mechanisms for these associations remain elusive. The large-scale meta-analysis of GWAS recently identified in Caucasians a CHD-associated locus at chromosome 6q23.2, a region containing the transcription factor TCF21 gene. TCF21 (Capsulin/Pod1/Epicardin is a member of the basic-helix-loop-helix (bHLH transcription factor family, and regulates cell fate decisions and differentiation in the developing coronary vasculature. Herein, we characterize a cis-regulatory mechanism by which the lead polymorphism rs12190287 disrupts an atypical activator protein 1 (AP-1 element, as demonstrated by allele-specific transcriptional regulation, transcription factor binding, and chromatin organization, leading to altered TCF21 expression. Further, this element is shown to mediate signaling through platelet-derived growth factor receptor beta (PDGFR-β and Wilms tumor 1 (WT1 pathways. A second disease allele identified in East Asians also appears to disrupt an AP-1-like element. Thus, both disease-related growth factor and embryonic signaling pathways may regulate CHD risk through two independent alleles at TCF21.

  2. Vertical and horizontal distribution of radionuclides (232Th, 238U and 40K) in sediment from Manjung coastal water area Perak, Malaysia

    International Nuclear Information System (INIS)

    Distribution of radionuclides from anthropogenic activities has been widely studied in marine coastal area. Due to rapid population growth and socio-economic development in Manjung area such as coal fired power plant, iron foundries, port development, waste discharged from factories and agriculture runoff may contribute to increase in pollution rate. The radioactive materials from anthropogenic activities could deteriorate the quality of the marine ecosystem and thus lead to possible radiological health risk to the population. Radionuclides (232Th, 238U and 40K) content in surface and profile sediment from Manjung coastal area was determined in this study. Radionuclides in sediment from seven locations were collected using sediment core sampling and measurements were carried out using Energy Dispersive X-ray Fluorescence (EDXRF) spectroscopy. The results show that the concentration of radionuclides in surface sediment and distribution trend of depth vertical profile sediment generally varies depending on locations. Enrichment factors (EF), geo-accumulation index (Igeo) and pollution index (PI) were applied to determine level of pollution of this study area. The radiological risks related to human exposure were evaluated based on external hazard index (Hex)

  3. Neutronic simulation of a research reactor core of (232Th, 235U)O2 fuel using MCNPX2.6 code

    Indian Academy of Sciences (India)

    Seyed Amir Hossein Feghhi; Marzieh Rezazadeh; Yachine Kadi; Claudio Tenreiro; Morteza Aref; Zohreh Gholamzadeh

    2013-01-01

    The small reactor design for the remote and less developed areas of the user countries should have simple features in view of the lack of infra-structure and resources. Many researchers consider long core life with no on-site refuelling activity as a primary feature for the small reactor design. Long core life can be achieved by enhancing internal conversion rate of fertile to fissile materials. For that purpose, thorium cycle can be adopted because a high fissile production rate of 233U converted from 232Th can be expected in the thermal energy region. A simple nuclear reactor core arranged 19 assemblies in hexagonal structure, using thorium-based fuel and heavy water as coolant and moderator was simulated using MCNPX2.6 code, aiming an optimized critical assembly. Optimized reflector thickness and gap between assemblies were determined to achieve minimum neutron leakage and void reactivity. The result was a more compact core, where assemblies were designed having 19-fuel pins in 1.25 pitch-to-diameter ratio. Optimum reflector thickness of 15 cm resulted in minimal neutron leakage in view of economic limitations. A 0.5 cm gap between assembles achieved more safety and 2.2% enrichment requirements. The present feasibility study suggests a thermal core of acceptable neutronic parameters to achieve a simple and safe core.

  4. Search for mass-symmetric ternary fission in the reactions {sup 14}N(53 A MeV)+{sup 197}Au and {sup 232}Th

    Energy Technology Data Exchange (ETDEWEB)

    Herbach, C.-M. E-mail: herbach@hmi.de; Hilscher, D.; Tishchenko, V.G.; Gippner, P.; Kamanin, D.V.; Oertzen, W. von; Ortlepp, H.-G.; Penionzhkevich, Yu.E.; Pyatkov, Yu.V.; Renz, G.; Schilling, K.D.; Strekalovsky, O.V.; Wagner, W.; Zhuchko, V.E

    2002-12-30

    Ternary fission of heavy hot composite systems with excitation energies of 1.5-2.5 MeV/amu has been studied in the reactions of {sup 14}N(53 A MeV) with {sup 197}Au and {sup 232}Th. The ternary yields have been explored as a function of the charge Z{sub L} of the lightest fragment: while Z{sub L} increases from 6 to 25, the cross sections decrease from 5 to 0.08 mb for N+Au and from 15 to 0.8 mb for N+Th. The velocity vector v{yields}{sub L} of the lightest fragment has been investigated in the rest frame of the other two heavier fragments. Two different components are observed: (i) an isotropic one with values of v{sub L} corresponding to the Coulomb repulsion from the combined heavier fragments before separation and, (ii) an anisotropic contribution with the lightest fragment emitted with lower v{sub L} perpendicular to the scission axis of the two heavier fragments. The latter component is distinguished from the isotropic one by an enhanced fraction of mass-symmetric ternary events and by up to 50 MeV lower total kinetic fragment energies. These features are indicative of a collinear stretched scission configuration, where the lightest fragment is positioned between the two heavier ones.

  5. Influence of different data tables on neutron induced reactions in quasi-infinite 238U and 232Th targets irradiated by protons with relativistic energy

    Science.gov (United States)

    Zhivkov, P.; Stoyanov, Ch; Tyutyunnikov, S.; Furman, W.

    2016-06-01

    The last decade saw the emergence of various theoretical analysis and developments of ADS (Accelerator Driving System). Different transport codes, nuclear models and nuclear cross sections have been used to predict and estimate the properties of ADS. The energy of the proton beam is supposed to range between 1 and 1.5 GeV, but some analyses suggest higher energy - up to 10 GeV. The recent papers examine the influence of the nuclear models on neutron induced reactions (n,f), (n,g), (n,xn), (n,el.) and (n,inel.). The experimental set-ups and the presumable ADS constructions consist of thousands of segments and details for example project Myrrha, Belgum [1]. The calculation of the above reactions depends on the neutron spectrum in each segment. There is a considerable difference in the size of these segments in ADS, which makes the estimation of the influence of the nuclear models and the cross sections on the integral number of neutron induced reactions more difficult. This article considers the influence of different cross section data tables on neutron induced reactions in 238U or 232Th targets. One nuclear model describing the high energy part of the nuclear interaction and various cross section data tagble (ENDF, ENDL, TENDL2014 and etc.) are used. All particles generated in the nuclear interaction process deposit their energy in the target volume. MCNP 6.1 transport code was used.

  6. 运河水系底质泥中~(226)Ra、~(232)Th、~(40)K 和~(137)Cs 含量的测定

    Institute of Scientific and Technical Information of China (English)

    程祺钧; 虎银秀; 巫柱中; 刘瑞源; 朱福敏

    1989-01-01

    通过对河水、底质泥、悬浮物以及生物样品中放射性核素含量的分析测量,可以了解水系放射性的主要来源以及放射性物质在环境介质中的迁移规律。1984年我们在长江水系放射性水平调查中,分别于1月份(枯水期)和7、8月份(丰水期)对运河水系8个站位的底质泥取样分析,用 Ge(Li)γ谱仪测定了底质泥中~(226)Ra (~(238)U)、~(232)Th、~(40)K 和~(137)Cs 含量,其中~(238)U 含量是按~(238)U-~(226)Ra 达放射性平衡推算的。

  7. Vertical and horizontal distribution of radionuclides ({sup 232}Th, {sup 238}U and {sup 40}K) in sediment from Manjung coastal water area Perak, Malaysia

    Energy Technology Data Exchange (ETDEWEB)

    Abdullah, Anisa, E-mail: coppering@ymail.com; Hamzah, Zaini; Wood, Ab. Khalik [Faculty of Applied Sciences, Universiti Teknologi MARA, 40450, Shah Alam, Selangor (Malaysia); Saat, Ahmad [Faculty of Applied Sciences, Universiti Teknologi MARA, 40450, Shah Alam, Selangor (Malaysia); Institute of Science, Universiti Teknologi MARA, 40450 Shah Alam, Selangor (Malaysia)

    2016-01-22

    Distribution of radionuclides from anthropogenic activities has been widely studied in marine coastal area. Due to rapid population growth and socio-economic development in Manjung area such as coal fired power plant, iron foundries, port development, waste discharged from factories and agriculture runoff may contribute to increase in pollution rate. The radioactive materials from anthropogenic activities could deteriorate the quality of the marine ecosystem and thus lead to possible radiological health risk to the population. Radionuclides ({sup 232}Th, {sup 238}U and {sup 40}K) content in surface and profile sediment from Manjung coastal area was determined in this study. Radionuclides in sediment from seven locations were collected using sediment core sampling and measurements were carried out using Energy Dispersive X-ray Fluorescence (EDXRF) spectroscopy. The results show that the concentration of radionuclides in surface sediment and distribution trend of depth vertical profile sediment generally varies depending on locations. Enrichment factors (EF), geo-accumulation index (I{sub geo}) and pollution index (PI) were applied to determine level of pollution of this study area. The radiological risks related to human exposure were evaluated based on external hazard index (H{sub ex})

  8. Concentration in activity of 137 Cs, 40 K, 232 Th, 226 Ra in waste deposits of the benefits of minerals in the State of Zacatecas

    International Nuclear Information System (INIS)

    The necessity to report the changes in the contained radionuclides in the terrestrial crust, or those deposited by the atomic tests around the world, becomes clear when observing the use of material of waste of those mines. With the purpose of quantifying the concentration in activity its were meet a series of waste samples in mines of the municipalities of Zacatecas, Fresnillo, Guadalupe and Veta Grande of the state of Zacatecas, Mexico. The analysis was carried out by gamma spectrometry with a HPGe detector with a resolution of 1.9 keV corresponding to an energy of 1.33 MeV calibrated in efficiency and energy by means of a certified standard multi nuclide in activity with identical geometry to that of the samples. The times of count are of 80000 seconds, with the purpose of to reduce the relative uncertainties and to define well the interest regions. The activity of 226 Ra and 232 Th is obtained through the one 214 Bi and 228 Ac respectively, the concentration was also measured in activity of the one 40 K and the 137 Cs in units of Bq kg-1. (Author)

  9. Calibration factors for determination of relativistic particle induced fission rates in natU, 235U, 232Th, natPb and 197Au foils

    International Nuclear Information System (INIS)

    Calibration factors w, for determination of fission rate in metallic foils of natU, 235U, 232Th, natPb and 197Au were determined for foils in contact with synthetic mica track detectors. Proton-induced fission at proton energies of 0.7 GeV and 1.5 GeV were used. Using our experimental results as well as those of the other authors, w for different foil-mica systems were determined. Two methods were used to calculate w, relative to the calibration factor for uranium-mica system, which has been obtained in a standard neutron field of energy 14.7 MeV. One of these methods requires the knowledge of the mean range of the fission fragments in the foils of interest and other method needs information on the values of the fission cross-sections at the required energies as well as the density of the tracks recorded in the track detectors in contact with the foil surfaces. The obtained w-values were compared with Monte Carlo calculations and good agreements were found. It is shown that a calibration factor obtained at low energy neutron induced fissions in uranium isotopes deviates only by less than 10% from those obtained at relativistic proton induced fissions.

  10. Simulation smuggling study for shielded sources of 235U, 238U, 232Th, 137Cs and 60Co by using γ-detection

    International Nuclear Information System (INIS)

    This work deals with gamma detection of shielded sources of 235U, 238U, 232Th, 137Cs and 60Co by using HpGe and NaI detectors through their main characteristic energies; 185.7 keV, (63, 1001), (583 and 911), 661.6 and (1173 and 1332) KeV respectively. These radioactive sources were individually hidden in containers of aluminum (Al), iron (Fe) and cupper (Cu) of different thicknesses; 3, 6, 9, 12, 15, 18 mm. Thin containers of lead (Pb) were also used with the same sources. The attenuation factor (I/I0), the ratio of radiation intensity with and without container or shield, was calculated for all the investigated γ-energies. The relationship between the attenuation factor and the studied thicknesses of the containers was given, depicted and discussed. Detection of the mixed sources shielded by different materials of different thicknesses was also carried out by using PDR-77 survey meter. The radiation levels were found to be within the natural background at 65cm distance from the shielded sources. Telescopic arm carrying 2x2 NaI and radiometer was also used. Generally, It can be concluded that smuggling of radioactive materials of low radioactivity can be done without detection by hiding them in containers or within scrap of Cu, Fe or even Al rather than using the conventional heavy lead shield. (author)

  11. Security and outcomes of interhopital transport of 232 critically ill children with congenital heart disease%探讨232例院际转运先天性心脏病危重患儿的安全性及其转归

    Institute of Scientific and Technical Information of China (English)

    孙跃玉; 昌艳军; 郭予雄; 钟敏泉; 何少茹

    2012-01-01

    Objectives To discuss the security of interhospital transport of critically ill children with congenital heart disease (CHD). Methods The clinical data, transport distance, duration and outcomes of 232 critically ill children with CHD who were transported from other hospitals in a period from August 2009 to July 2011 were analyzed retrospectively. Results Among 232 critically ill children with CHD, there were 152 males and 80 females;their ages ranged from 1 month to 12 years old (median 5 months); weights ranged from 2.5 kg to 25 kg (median 5.5 kg) ; transport durations ranged from 20 min to 990 min (median 156 min); transport distances ranged from 74 km to 620 km (median 204 km), and 47.2% of them were transported from hospitals 100 km to 200 km away (median 148 km). None of the patients died and all of them were hospitalized in the pediatric intensive care unit (PICU) of Guangdong General Hospital. There were 56 (24.1%) children required ventilation during transport. In the end, 220 patients were cured or improved, 9 of them gave up treatment, 3 of them died. Conclusions A specialized retrieval team with adequate preparation before transport, close observation and monitoring on the way can effectively lower mortality and disability rates of critically ill children with CHD and improve the security and outcomes of interhospital transport.%目的 探讨先天性心脏病危重症患儿院际转运的安全性.方法 回顾性分析2009年8月至2011年7月院际转运的232例先天性心脏病危重症患儿的转运前、中和到儿科监护病房(pediatric intensive care unit,PICU)后的临床资料、转运距离、时间和患儿的转归.结果 232例患儿,男152例,女80例;年龄1个月~12岁,中位年龄5个月;体质量2.5~25 kg,中位体质量5.5 kg;转运花费时间20~990 min,中位时间156 min;转运距离是74~620 km,中位距离204 km,其中47.2%的患儿转运距离100~200 km,中位距离148 km.转运过程中需要

  12. How to Do Well the Job of Prevention and Cure of Psychosis in the Community-Add the Investigation and Analysis of 232 Cases of Psychosis%如何做好精神病病人社区防治工作--附232例精神病病人的调查分析

    Institute of Scientific and Technical Information of China (English)

    康健; 林玲

    2002-01-01

    通过对天河南街社区中232例精神病病人的调查分析,发现在各类精神病病人中,阿尔采末病的患病人数最多,其次为精神分裂症.无职业者患病率最高;较低文化层次的人群患病率也较高.讨论了精神病发病与社会环境心理因素的关系,以及提出了做好精神病病人社区防治工作的几点措施.

  13. Cluster spin glass behavior of Li[Li(1/3-x/3)Mn(2/3-2x/3)Cox]O2(x=0.1)%Li[Li(1/3-x/3)Mn(2/3-2x/3)Cox]O2(x=O.1)的团簇自旋玻璃态行为

    Institute of Scientific and Technical Information of China (English)

    高春歌; 王丽萍; 陈红; 王春忠

    2011-01-01

    采用柠檬酸盐法制备了六方层状结构的Li[Li(1/3-x/3)Mn(2/3-2x/3)Cox]O2(x=0.1)材料.体系在高温区呈现顺磁态,通过拟合Curie-Weiss定律得到Curie和Weiss常数分别为1.70(2)m3 K/mol和-22(3)K.该材料的磁化率曲线在低温区表现出不可逆转变行为,并且这种不可逆转变行为也受到外加磁场的调制.结合Almeida-Thouless(AT)线分析,可以确定Li[Li0.3Mn0.6Co0.1]O2呈现团簇自旋玻璃态行为.%Li[Li(1/3-x/3)Mn(2/3-2X/3)Cox]O2(x = 0. 1) was prepared by citrate precursor method and show paramagnetism during high-temperature region. By fitting Curie-Weiss law, the Curie and Weiss constant are obtained to be 1. 70(2)m3 K/mol and - 22(3) K,respectively. The susceptibility shows irreversibility behavior at low temperature and this irreversibility behavior is suppressed by applied fields. Together with Almeida-Thouless (AT), Cluster spin glass behavior is suggested to be the ground state of Li[Li0.3Mn0.6Co0.1]O2.

  14. Determination of the neutron capture cross sections of 232Th at 14.1 MeV and 14.8 MeV using the neutron activation method

    CERN Document Server

    Lan, Chang-Lin; Peng, Meng; Lv, Tao; Yao, Ze-en; Chen, Jin-Gen; Kong, Xiang-Zhong

    2016-01-01

    The 232Th(n,{\\gamma})233Th neutron capture reaction cross sections were measured at average neutron energies of 14.1 MeV and 14.8 MeV using the activation method. The neutron flux was determined using the monitor reaction 27Al(n,{\\alpha})24Na. The induced gamma-ray activities were measured using a low background gamma ray spectrometer equipped with a high resolution HPGe detector. The experimentally determined cross sections were compared with the literatures data, evaluated data of ENDF/B-VII, JENDL-4.0, and CENDL-3.1. The Excitation functions of 232Th(n,{\\gamma}) reaction were also calculated theoretically using the TALYS 1.6 computer code.

  15. Measurement of 238U and 232Th in Petrol, Gas-oil and Lubricant Samples by Using Nuclear Track Detectors and Resulting Radiation Doses to the Skin of Mechanic Workers.

    Science.gov (United States)

    Misdaq, M A; Chaouqi, A; Ouguidi, J; Touti, R; Mortassim, A

    2015-10-01

    Workers in repair shops of vehicles (cars, buses, truck, etc.) clean carburetors, check fuel distribution, and perform oil changes and greasing. To explore the exposure pathway of (238)U and (232)Th and its decay products to the skin of mechanic workers, these radionuclides were measured inside petrol, gas-oil, and lubricant material samples by means of CR-39 and LR-115 type II solid state nuclear track detectors (SSNTDs), and corresponding annual committed equivalent doses to skin were determined. The maximum total equivalent effective dose to skin due to the (238)U and (232)Th series from the application of different petrol, gas-oil, and lubricant samples by mechanic workers was found equal to 1.2 mSv y(-1) cm(-2). PMID:26313584

  16. 放射性核素土壤-植物吸收与钍、镭富集植物的发现%Uptake of Radionuclides from Soil to Plant and the Discovery of 226Ra, 232Th Hyperaccumulator

    Institute of Scientific and Technical Information of China (English)

    张志强; 陈迪云; 宋刚; 岳玉美

    2011-01-01

    11 sorts of plant samples and corresponding soil samples were collected in Conghua and Taishan, Pearl River Delta. The specific activity of 238U、226Ra、232Th and 40K of samples were investigated by using HPGe-γ-ray spectra analysis. The results showed that the average specific activity of 238U, 226Ra, 232Th and 40K in soil samples were 151.8, 146. 3, 226. 6, 665.5 Bq/kg, which were higher than the average values of China and the world. The concentration of 238U in all sort of plants are very low and most of them are lower than detection limit, while the values of 226Ra, 232Th and 4OK were high. The contents of 226Ra and 232Th in Dicranopteris dichotoma were the highest, whose average specific activity is 285.9, 986. 2 Bq/kg respectively. The average bioconcentration factors (BFs)of 226Ra,232Th of Dicranopteris dichotoma were 2. 20, 4.23, respectively, the other 10 sort of plants have BFs of 226Ra, 232Th were in the range of 10 -1 -10-2. The bioconcentration factors and the translocation factors of 226Ra, 232Th of Dicranopteris dichotoma were all bigger than 1, so Dicranopteris dichotoma can be defined as hyperaccumulator of 226Ra and 232Th.%对采集珠江三角洲从化、台山等地的11种植物以及对应的土壤样品,采用HPGe-y能谱分析了其中的天然放射性核素U、Ra、Th和K的比活度,结果表明,土壤样品中U、Ra、Th和K的平均含量为151.8、146.3、226.6和665.5Bq/kg,高于我国和世界的平均值,植物样品中的U含量较低,大多数样品低于检出限,而Ra、Th和K的平均含量相对较高.铁芒萁(Dicranopteris dichotoma)样品中Ra、Th含量最高,平均值分别为285.9 Bq/kg、968.5 Bq/kg,对应的生物富集系数(bioconcentration factor)的平均值为2.20、4.23,而其它10种植物Ra、Th的生物富集系数均在10~10的范围.铁芒萁Ra和Th的富集系数和转移系数(translocation factor)都大于1,可以认为是Ra和Th的超富集植物.

  17. Use of electrodeposition for sample preparation and rejection rate prediction for assay of electroformed ultra high purity copper for 232Th and 238U prior to inductively coupled plasma mass spectrometry (ICP/MS)

    International Nuclear Information System (INIS)

    The search for neutrinoless double beta decay in 76Ge has driven the need for ultra-low background Ge detectors shielded by electroformed copper of ultra-high radiopurity (232Th and 238U into the plating bath simulates low purity copper and allows for the calculation of the electrochemical rejection rate of thorium and uranium in the electroplating system. This rejection value will help to model plating bath chemistry. (author)

  18. Development of sequential analytical method for the determination of U-238, U-234, Th-232, Th-230, Th-228, Ra-226 and Ra-228 and its application in mineral waters

    International Nuclear Information System (INIS)

    A sequential analytical method for the determination of U-238, U-234, Th-232, Th-230, Th-228, Ra-226 and Ra-228 in environmental samples and applied to the analysis of mineral waters is studied. Thorium isotopes are coprecipitated with lanthanium fluoride before counting in alpha spectrometer, the uranium isotopes are determined by alpha spectrometry following extraction with TOPO onto a polymenic membrane. Radium-226 is determined with the radom emanation technique. (M.J.C.)

  19. Association of a lysine-232/alanine polymorphism in a bovine gene encoding acyl-CoA:diacylglycerol acyltransferase (DGAT1) with variation at a quantitative trait locus for milk fat content.

    Science.gov (United States)

    Winter, Andreas; Krämer, Wolfgang; Werner, Fabian A O; Kollers, Sonja; Kata, Srinivas; Durstewitz, Gregor; Buitkamp, Johannes; Womack, James E; Thaller, Georg; Fries, Ruedi

    2002-07-01

    DGAT1 encodes diacylglycerol O-acyltransferase (EC ), a microsomal enzyme that catalyzes the final step of triglyceride synthesis. It became a functional candidate gene for lactation traits after studies indicated that mice lacking both copies of DGAT1 are completely devoid of milk secretion, most likely because of deficient triglyceride synthesis in the mammary gland. Our mapping studies placed DGAT1 close to the region of a quantitative trait locus (QTL) on bovine chromosome 14 for variation in fat content of milk. Sequencing of DGAT1 from pooled DNA revealed significant frequency shifts at several variable positions between groups of animals with high and low breeding values for milk fat content in different breeds (Holstein-Friesian, Fleckvieh, and Braunvieh). Among the variants was a nonconservative substitution of lysine by alanine (K232A), with the lysine-encoding allele being associated with higher milk fat content. Haplotype analysis indicated the lysine variant to be ancestral. Two animals that were typed heterozygous (Qq) at the QTL based on marker-assisted QTL-genotyping were heterozygous for the K232A substitution, whereas 14 animals that are most likely qq at the QTL were homozygous for the alanine-encoding allele. An independent association study in Fleckvieh animals confirmed the positive effect of the lysine variant on milk fat content. We consider the nonconservative K232A substitution to be directly responsible for the QTL variation, although our genetic studies cannot provide formal proof.

  20. Development of an analytical method for the determination of U-238, U-234, Th-232, Th-230, Th-228, Ra-228, Ra-226, Pb-210 and Po-210 and its application on environmental samples

    International Nuclear Information System (INIS)

    A comparison between the environmental impact by nuclear facilities with the burden suffered from natural radioactivity calls for studying the long-lived radionuclides of the U-238 and Th-232 decay series U-238, U-234, Th-232, Th-230, Th-228, Ra-228, Ra-226, Pb-210 and Po-210. This work describes the development of a fast isotope dilution analysis method allowing to separate with one sample solution U, Th, Ra, Pb and Po both from each other and, at the same time, from the matrix. To test its applicability, the method was used with samples consisting of soil, sediments, plants, water, carbon and air dust filter. The detection limit for the chemical yield attained of approx. 70% was 0.27 mBq per sample for Th-232, Th-230, Th-228, U-238, U-234 and Po-210. The detection limit for Pb-210 was 10 mBq per sample. On account of the influence by Ra-226 in the Ra-228 measurement and vice versa the detection limit is a function of the Ra-226 and Ra-228 concentrations, respectively, in the sample. The detection limits for the pure nuclides are 0.9 mBq per sample and 10 mBq per sample, respectively, for Ra-226 and Ra-228. (orig./HP)