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Sample records for upper tropospheric zonal

  1. EOF analysis of COSMIC observations on the global zonal mean temperature structure of the Upper Troposphere and Lower Stratosphere from 2007 to 2013

    Science.gov (United States)

    Salinas, Cornelius Csar Jude H.; Chang, Loren C.

    2018-06-01

    This work presents the results of a Conventional Empirical Orthogonal Function Analysis on daily global zonal mean temperature profiles in the Upper Troposphere and Lower Stratosphere (15-35 km), as measured by the FORMOSAT-3/COSMIC mission from January 2007 to June 2013. For validation, results were compared with ERA-Interim reanalysis. Results show that, the leading global EOF mode (27%) from COSMIC is consistent with temperature anomalies due to the tropical cooling associated with boreal winter Sudden Stratospheric Warmings (SSW). The second global EOF mode from COSMIC (15.3%) is consistent with temperature anomalies due to the Quasi-biennial Oscillation (QBO). The third global mode from COSMIC (10.9%) is consistent with temperature anomalies due to the El Nino Southern Oscillation. This work also shows that the second northern hemisphere EOF mode from COSMIC (16.8%) is consistent with temperature anomalies due Rossby-wave breaking (RWB) which is expected to only be resolved by a high vertical and temporal resolution dataset like COSMIC. Our work concludes that the use of a high vertical and temporal resolution dataset like COSMIC yields non-seasonal EOF modes that are consistent with relatively more intricate temperature anomalies due to the SSW, QBO, ENSO and RWB.

  2. Changes to Saturn's zonal-mean tropospheric thermal structure after the 2010-2011 northern hemisphere storm

    Energy Technology Data Exchange (ETDEWEB)

    Achterberg, R. K.; Hesman, B. E. [Department of Astronomy, University of Maryland, College Park, MD 20742 (United States); Gierasch, P. J.; Conrath, B. J. [Department of Astronomy, Cornell University, Ithaca, NY 14853 (United States); Fletcher, L. N. [Atmospheric Oceanic and Planetary Physics, University of Oxford, Clarenden Laboratory, Parks Road, Oxford OX1 3PU (United Kingdom); Bjoraker, G. L.; Flasar, F. M., E-mail: Richard.K.Achterberg@nasa.gov [Planetary Systems Laboratory NASA/GSFC, Greenbelt, MD 20771 (United States)

    2014-05-10

    We use far-infrared (20-200 μm) data from the Composite Infrared Spectrometer on the Cassini spacecraft to determine the zonal-mean temperature and hydrogen para-fraction in Saturn's upper troposphere from observations taken before and after the large northern hemisphere storm in 2010-2011. During the storm, zonal mean temperatures in the latitude band between approximately 25°N and 45°N (planetographic latitude) increased by about 3 K, while the zonal mean hydrogen para-fraction decreased by about 0.04 over the same latitudes, at pressures greater than about 300 mbar. These changes occurred over the same latitude range as the disturbed cloud band seen in visible images. The observations are consistent with low para-fraction gas being brought up from the level of the water cloud by the strong convective plume associated with the storm, while being heated by condensation of water vapor, and then advected zonally by the winds near the plume tops in the upper troposphere.

  3. RELATIONSHIPS BETWEEN ZONAL WIND ANOMALIES IN HIGH AND LOW TROPOSPHERE AND ANNUAL FREQUENCY OF NW PACIFIC TROPICAL CYCLONES

    Institute of Scientific and Technical Information of China (English)

    GONG Zhen-song; HE Min

    2007-01-01

    Relationships between large-scale zonal wind anomalies and annual frequency of NW Pacific tropical cyclones and possible mechanisms are investigated with the methods of correlation and composition.It is indicated that when △ U200-△U850 >0 in the eastern tropical Pacific and △ U200- △U850 <0 in western tropical Pacific, the Walker cell is stronger in the Pacific tropical region and the annual frequency of NW Pacific tropical cyclone are above normal. In the years with zonal wind anomalies, the circulation of high and low troposphere and the vertical motions in the troposphere have significant characteristics. In the time scale of short-range climate prediction, zonal wind anomalies in high and low troposphere are useful as a preliminary signal of the annual frequency prediction of NW Pacific tropical cyclones.

  4. Factors controlling upper tropospheric relative humidity

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    B. Kärcher

    2004-03-01

    Full Text Available Factors controlling the distribution of relative humidity in the absence of clouds are examined, with special emphasis on relative humidity over ice (RHI under upper tropospheric and lower stratospheric conditions. Variations of temperature are the key determinant for the distribution of RHI, followed by variations of the water vapor mixing ratio. Multiple humidity modes, generated by mixing of different air masses, may contribute to the overall distribution of RHI, in particular below ice saturation. The fraction of air that is supersaturated with respect to ice is mainly determined by the distribution of temperature. The nucleation of ice in cirrus clouds determines the highest relative humdity that can be measured outside of cirrus clouds. While vertical air motion and ice microphysics determine the slope of the distributions of RHI, as shown in a separate study companion (Haag et al., 2003, clouds are not required to explain the main features of the distributions of RHI below the ice nucleation threshold. Key words. Atmospheric composition and structure (pressure, density and temperature; troposphere – composition and chemistry; general or miscellaneous

  5. Factors controlling upper tropospheric relative humidity

    Directory of Open Access Journals (Sweden)

    B. Kärcher

    2004-03-01

    Full Text Available Factors controlling the distribution of relative humidity in the absence of clouds are examined, with special emphasis on relative humidity over ice (RHI under upper tropospheric and lower stratospheric conditions. Variations of temperature are the key determinant for the distribution of RHI, followed by variations of the water vapor mixing ratio. Multiple humidity modes, generated by mixing of different air masses, may contribute to the overall distribution of RHI, in particular below ice saturation. The fraction of air that is supersaturated with respect to ice is mainly determined by the distribution of temperature. The nucleation of ice in cirrus clouds determines the highest relative humdity that can be measured outside of cirrus clouds. While vertical air motion and ice microphysics determine the slope of the distributions of RHI, as shown in a separate study companion (Haag et al., 2003, clouds are not required to explain the main features of the distributions of RHI below the ice nucleation threshold.

    Key words. Atmospheric composition and structure (pressure, density and temperature; troposphere – composition and chemistry; general or miscellaneous

  6. Longitudinal differences and inter-annual variations of zonal wind in the tropical stratosphere and troposphere

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    Reddy, C. A.; Raghava Reddi, C.

    1986-12-01

    A quantitative assessment has been made of the longitude-dependent differences and the interannual variations of the zonal wind components in the equatorial stratosphere and troposphere, from the analysis of rocket and balloon data for 1979 and 1980 for three stations near ±8.5° latitude (Ascension Island at 14.4°W, Thumba at 76.9°E and Kwajalein at 67.7°E) and two stations near 21.5° latitude (Barking Sands at 159.6°W and Balasore at 86.9°E). The longitude-dependent differences are found to be about 10-20 m s -1 (amounting to 50-200% in some cases) for the semi-annual oscillation (SAO) and the annual oscillation (AO) amplitudes, depending upon the altitude and latitude. Inter-annual variations of about 10 m s -1 also exist in both oscillations. The phase of the SAO exhibits an almost 180° shift at Kwajalein compared to that at the other two stations near 8.5°, while the phase of the AO is independent of longitude, in the stratosphere. The amplitude and phase of the quasi-biennial oscillation (QBO) are found to be almost independent of longitude in the 18-38 km range, but above 40 km height the QBO amplitude and phase have different values in different longitude sectors for the three stations near ±8.5° latitude. The mean zonal wind shows no change from 1979 to 1980, but in the troposphere at 8.5° latitude strong easterlies prevail in the Indian zone, in contrast to the westerlies at the Atlantic and Pacific stations.

  7. Retrieval of global upper tropospheric and stratospheric formaldehyde (H2CO distributions from high-resolution MIPAS-Envisat spectra

    Directory of Open Access Journals (Sweden)

    G. P. Stiller

    2008-02-01

    Full Text Available The Fourier transform spectrometer MIPAS (Michelson Interferometer for Passive Atmospheric Sounding on Envisat measures infrared emission of the Earth's atmosphere in a limb viewing mode. High spectral resolution measurements of MIPAS are sensitive to formaldehyde from the upper troposphere to the stratopause. Single profile retrievals of formaldehyde are dominated by a 60% noise error; however zonal mean values for 30 days of data during 8 September 2003 and 1 December 2003 reduces this error by a factor of 20 or more. The number of degrees of freedom for single profile retrieval ranges from 2 to 4.5 depending on latitude and number of cloud-free tangent altitudes. In the upper tropical troposphere zonal mean values of about 70 parts per trillion by volume (pptv were found, which have been attributed to biomass burning emissions. In the stratosphere, formaldehyde values are determined by photochemical reactions. In the upper tropical stratosphere, formaldehyde zonal mean maximum values can reach 130 pptv. Diurnal variations in this region can be up to 50 pptv. Comparisons with other satellite instruments show generally good agreement in the region of upper troposphere and lower stratosphere as well as in the upper stratosphere.

  8. A simple climatology of westerly jet streams in global reanalysis datasets part 1: mid-latitude upper tropospheric jets

    Science.gov (United States)

    Rikus, Lawrie

    2018-04-01

    A simple closed contour object identification scheme has been applied to the zonal mean monthly mean zonal wind fields from nine global reanalysis data sets for 31 years of the satellite era (1979-2009) to identify objects corresponding to westerly jet streams. The results cluster naturally into six individual jet streams but only the mid-latitude upper-tropospheric jets are considered here. The time series of the jet properties from all reanalyses are decomposed into seasonal means and anomalies, and correlations between variables are evaluated, with the aim of identifying robust features which can form the basis of evaluation metrics for climate model simulations of the twentieth century. There is substantial agreement between all the reanalyses for all jet properties although there are some systematic differences with particular data sets. Some of the results from the object identification applied to the reanalyses are used in a simple example of a model evaluation score for the zonal mean jet seasonal cycle.

  9. Stratospheric ozone transboundary transport to upper troposphere North Africa

    CSIR Research Space (South Africa)

    Ture, K

    2011-09-01

    Full Text Available will identify the causes and sources of MOZAIC ozone enhancements at upper tropospheric North Africa (20-350 N). In addition the paper will address the modes of transport of ozone rich airmass sampled by MOZAIC at mid latitude and North Africa....

  10. Comparisons of Upper Tropospheric Humidity Retrievals from TOVS and METEOSAT

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    Escoffier, C.; Bates, J.; Chedin, A.; Rossow, W. B.; Schmetz, J.

    1999-01-01

    Two different methods for retrieving Upper Tropospheric Humidities (UTH) from the TOVS (TIROS Operational Vertical Sounder) instruments aboard NOAA polar orbiting satellites are presented and compared. The first one, from the Environmental Technology Laboratory, computed by J. Bates and D. Jackson (hereafter BJ method), estimates UTH from a simplified radiative transfer analysis of the upper tropospheric infrared water vapor channel at wavelength measured by HIRS (6.3 micrometer). The second one results from a neural network analysis of the TOVS (HIRS and MSU) data developed at, the Laboratoire de Meteorologie Dynamique (hereafter the 3I (Improved Initialization Inversion) method). Although the two methods give very similar retrievals in temperate regions (30-60 N and S), an absolute bias up to 16% appears in the convective zone of the tropics. The two datasets have also been compared with UTH retrievals from infrared radiance measurements in the 6.3 micrometer channel from the geostationary satellite METEOSAT (hereafter MET method). The METEOSAT retrievals are systematically drier than the TOVS-based results by an absolute bias between 5 and 25%. Despite the biases, the spatial and temporal correlations are very good. The purpose of this study is to explain the deviations observed between the three datasets. The sensitivity of UTH to air temperature and humidity profiles is analysed as are the clouds effects. Overall, the comparison of the three retrievals gives an assessment of the current uncertainties in water vapor amounts in the upper troposphere as determined from NOAA and METEOSAT satellites.

  11. The Impact of Upper Tropospheric Humidity from Microwave Limb Sounder on the Midlatitude Greenhouse Effect

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    Hu, Hua; Liu, W. Timothy

    1998-01-01

    This paper presents an analysis of upper tropospheric humidity, as measured by the Microwave Limb Sounder, and the impact of the humidity on the greenhouse effect in the midlatitudes. Enhanced upper tropospheric humidity and an enhanced greenhouse effect occur over the storm tracks in the North Pacific and North Atlantic. In these areas, strong baroclinic activity and the large number of deep convective clouds transport more water vapor to the upper troposphere, and hence increase greenhouse trapping. The greenhouse effect increases with upper tropospheric humidity in areas with a moist upper troposphere (such as areas over storm tracks), but it is not sensitive to changes in upper tropospheric humidity in regions with a dry upper troposphere, clearly demonstrating that there are different mechanisms controlling the geographical distribution of the greenhouse effect in the midlatitudes.

  12. New Particle Formation in the Mid-Latitude Upper Troposphere

    Science.gov (United States)

    Axisa, Duncan

    Primary aerosol production due to new particle formation (NPF) in the upper troposphere and the impact that this might have on cloud condensation nuclei (CCN) concentration can be of sufficient magnitude to contribute to the uncertainty in radiative forcing. This uncertainty affects our ability to estimate how sensitive the climate is to greenhouse gas emissions. Therefore, new particle formation must be accurately defined, parametrized and accounted for in models. This research involved the deployment of instruments, data analysis and interpretation of particle formation events during the Mid-latitude Airborne Cirrus Properties Experiment (MACPEX) campaign. The approach combined field measurements and observations with extensive data analysis and modeling to study the process of new particle formation and growth to CCN active sizes. Simultaneous measurements of O3, CO, ultrafine aerosol particles and surface area from a high-altitude research aircraft were used to study tropospheric-stratospheric mixing as well as the frequency and location of NPF. It was found that the upper troposphere was an active region in the production of new particles by gas-to-particle conversion, that nucleation was triggered by convective clouds and mixing processes, and that NPF occurred in regions with high relative humidity and low surface area. In certain cases, mesoscale and synoptic features enhanced mixing and facilitated the formation of new particles in the northern mid-latitudes. A modeling study of particle growth and CCN formation was done based on measured aerosol size distributions and modeled growth. The results indicate that when SO2 is of sufficient concentration NPF is a significant source of potential CCN in the upper troposphere. In conditions where convective cloud outflow eject high concentrations of SO2, a large number of new particles can form especially in the instance when the preexisting surface area is low. The fast growth of nucleated clusters produces a

  13. Sub-seasonal temperature variability in the tropical upper troposphere and lower stratosphere observed with GPS radio occultation

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    Scherllin-Pirscher, Barbara; Randel, William J.; Kim, Joowan

    2017-04-01

    We investigate sub-seasonal temperature variability in the tropical upper troposphere and lower stratosphere (UTLS) region using daily gridded fields of GPS radio occultation measurements. The unprecedented vertical resolution (from about 100 m in the troposphere to about 1.5 km in the stratosphere) and high accuracy and precision (0.7 K to 1 K between 8 km and 25 km) make these data ideal for characterizing temperature oscillations with short vertical wavelengths. Long-term behavior of sub-seasonal temperature variability is investigated using the entire RO record from January 2002 to December 2014 (13 years of data). Transient sub-seasonal waves including eastward-propagating Kelvin waves (isolated with space-time spectral analysis) dominate large-scale zonal temperature variability in the tropical tropopause region and in the lower stratosphere. Above 20 km, Kelvin waves are strongly modulated by the quasi-biennial oscillation (QBO). Enhanced wave activity can be found during the westerly shear phase of the QBO. In the tropical tropopause region, however, sub-seasonal waves are highly transient in time. Several peaks of Kelvin-wave activity coincide with short-term fluctuations in tropospheric deep convection, but other episodes are not evidently related. Also, there are no obvious relationships with zonal winds or stability fields near the tropical tropopause. Further investigations of convective forcing and atmospheric background conditions along the waves' trajectories are needed to better understand sub-seasonal temperature variability near the tropopause. For more details, see Scherllin-Pirscher, B., Randel, W. J., and Kim, J.: Tropical temperature variability and Kelvin-wave activity in the UTLS from GPS RO measurements, Atmos. Chem. Phys., 17, 793-806, doi:10.5194/acp-17-793-2017, 2017. http://www.atmos-chem-phys.net/17/793/2017/acp-17-793-2017.html

  14. Water vapour and ozone profiles in the midlatitude upper troposphere

    Directory of Open Access Journals (Sweden)

    G. Vaughan

    2005-01-01

    Full Text Available We present an investigation of upper tropospheric humidity profiles measured with a standard radiosonde, the Vaisala RS80-A, and a commercial frost-point hygrometer, the Snow White. Modifications to the Snow White, to enable the mirror reflectivity and Peltier cooling current to be monitored during flight, were found to be necessary to determine when the instrument was functioning correctly; a further modification to prevent hydrometeors entering the inlet was also implemented. From 23 combined flights of an ozonesonde, radiosonde and Snow White between September 2001 and July 2002, clear agreement was found between the two humidity sensors, with a mean difference of <2% in relative humidity from 2 to 10km, and 2.2% between 10 and 13km. This agreement required a correction to the radiosonde humidity, as described by Miloshevich et al. (2001. Using this result, the dataset of 324 ozonesonde/RS80-A profiles measured from Aberystwyth between 1991 and 2002 was examined to derive statistics for the distribution of water vapour and ozone. Supersaturation with respect to ice was frequently seen at the higher levels - 24% of the time in winter between 8 and 10km. The fairly uniform distribution of relative humidity persisted to 120% in winter, but decreased rapidly above 100% in summer.

  15. Observational evidence for aerosols increasing upper tropospheric humidity

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    L. Riuttanen

    2016-11-01

    Full Text Available Aerosol–cloud interactions are the largest source of uncertainty in the radiative forcing of the global climate. A phenomenon not included in the estimates of the total net forcing is the potential increase in upper tropospheric humidity (UTH by anthropogenic aerosols via changes in the microphysics of deep convection. Using remote sensing data over the ocean east of China in summer, we show that increased aerosol loads are associated with an UTH increase of 2.2 ± 1.5 in units of relative humidity. We show that humidification of aerosols or other meteorological covariation is very unlikely to be the cause of this result, indicating relevance for the global climate. In tropical moist air such an UTH increase leads to a regional radiative effect of 0.5 ± 0.4 W m−2. We conclude that the effect of aerosols on UTH should be included in future studies of anthropogenic climate change and climate sensitivity.

  16. Observations of peroxyacetyl nitrate (PAN) in the upper troposphere by the Atmospheric Chemistry Experiment Fourier Transform Spectrometer (ACE-FTS)

    Science.gov (United States)

    Tereszchuk, K. A.; Moore, D. P.; Harrison, J. J.; Boone, C. D.; Park, M.; Remedios, J. J.; Randel, W. J.; Bernath, P. F.

    2013-01-01

    Peroxyacetyl nitrate (CH3CO·O2NO2, abbreviated as PAN) is a trace molecular species present in the troposphere and lower stratosphere due primarily to pollution from fuel combustion and the pyrogenic outflows from biomass burning. In the lower troposphere, PAN has a relatively short life-time and is principally destroyed within a few hours through thermolysis, but it can act as a reservoir and carrier of NOx in the colder temperatures of the upper troposphere where UV photolysis becomes the dominant loss mechanism. Pyroconvective updrafts from large biomass burning events can inject PAN into the upper troposphere and lower stratosphere (UTLS), providing a means for the long-range transport of NOx. Given the extended lifetimes at these higher altitudes, PAN is readily detectable via satellite remote sensing. A new PAN data product is now available for the Atmospheric Chemistry Experiment Fourier Transform Spectrometer (ACE-FTS) Version 3.0 data set. We report measurements of PAN in Boreal biomass burning plumes recorded during the Quantifying the impact of BOReal forest fires on Tropospheric oxidants over the Atlantic using Aircraft and Satellites (BORTAS) campaign. The retrieval method employed and errors analysis are described in full detail. The retrieved volume mixing ratio (VMR) profiles are compared to coincident measurements made by the Michelson Interferometer for Passive Atmospheric Sounding (MIPAS) instrument on the European Space Agency (ESA) ENVIronmental SATellite (ENVISAT). Three ACE-FTS occultations containing measurements of Boreal biomass burning outflows, recorded during BORTAS, were identified as having coincident measurements with MIPAS. In each case, the MIPAS measurements demonstrated good agreement with the ACE-FTS VMR profiles for PAN. The ACE-FTS PAN data set is used to obtain zonal mean distributions of seasonal averages from ~5 to 20 km. A strong seasonality is clearly observed for PAN concentrations in the global UTLS. Since the

  17. Aqueous aerosol may build up large upper tropospheric ice supersaturation

    Science.gov (United States)

    Bogdan, Anatoli; Molina, Mario J.

    2010-05-01

    Keywords: ice supersaturation, upper tropospheric cirrus clouds, freezing of aqueous aerosol. Observations often reveal enhanced and persistent upper tropospheric (UT) ice supersaturation, Si up to 100%, independently of whether cirrus ice clouds are present or not (Krämer et al., 2009; Lawson et al., 2008). However, a water activity criterion (WAC) (Koop et al., 2000) does not allow the formation of Si > ~67% by the homogeneous freezing of aqueous droplets even at the lowest atmospheric temperature of ~185 K. For aqueous aerosol the WAC predicts the existence of a so called homogeneous ice nucleation threshold which, being expressed as Si, is between ~52 and 67% in the temperature range of ~220 - 185 K. The nature of the formation of large Si remains unclear. Since water vapor is the dominant greenhouse gas it is important to know the nature of the accumulation and persistence of water vapor in the UT. We studied the freezing behavior of micrometer-scaled 3-, 4-, and 5-component droplets, which contain different weight fractions of H2O, H2SO4, HNO3, (NH4)2SO4, (NH4)HSO4, NH4NO3, and (NH4)3H(SO4)2. The study was performed between 133 and 278 K at cooling rates of 3, 0.1, and 0.05 K/min using differential scanning calorimetry (DSC) (Bogdan and Molina, 2010). The cooling rates of 0.1 and 0.05 K/min (6 and 3 K/h) are similar to the smallest reported synoptic temperature change of ~2 K/h (Carslaw et al., 1998). Using the measured freezing temperature of ice, Ti, and the thermodynamic E-AIM model of the system of H+ - NH4+ - SO42-- NO3-- H2O (Clegg et al., 1998), we calculated the corresponding clear-sky Si which would be built up immediately prior to the formation of ice cirrus clouds by the homogeneous freezing of aqueous aerosol of similar composition. We found that our calculated values of Si are both larger and smaller than the homogeneous ice nucleation threshold. For example, for the droplets of compositions of 15/10 and 20/10 wt % (NH4)3H(SO4)2/H2SO4, which

  18. Relationship between changes in the upper and lower tropospheric water vapor: A revisit

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    Yang, M.; Sun, D. Z.; Zhang, G. J.

    2017-12-01

    Upper tropospheric water vapor response to enhanced greenhouse gas forcing is as important as the lower tropospheric water vapor response in determining climate sensitivity. Early studies using older versions of climate models have suggested that the upper- and lower-troposphere water vapor changes are more strongly coupled in the climate models than in the observations. Here we reexamine this issue using a state-of-the-art climate model—the NCAR community model CAM5. Specifically, we have calculated the correlations between interannual variations of specific humidity in all levels of the troposphere with that at the surface in CAM5 and in the observations (as represented by the updated ERA-Interim and NCEP reanalysis). It is found that the previously noted biases in how strongly upper tropospheric water vapor and lower troposphere water vapor are linked still exist in CAM5—the change in the tropical averaged upper tropospheric water vapor is more strongly correlated with the change in the surface. However, this bias disappears in the averaged correlation obtained by averaging the point-by-point correlations over the tropics. The spatial pattern of the point-by-point correlations reveals that the better agreement between the model and the observations is related to the opposite model biases in different regions: the correlation is weaker in the model in the western Pacific, but stronger in the central and eastern Pacific. Further analysis of precipitation fields suggests that the weaker (stronger) coupling between tropospheric water vapor and surface moisture over western (central-eastern) Pacific in model is related to weaker (stronger) simulated convective activities in these regions. More specifically, during El Nino, the model has excessive deep convection in the central Pacific, but too littler deep convection in western Pacific. Implications of the results are discussed in the context of climate change as well as in the context of how to improve the model

  19. Hydrogen Radicals, Nitrogen Radicals, and the Production of O3 in the Upper Troposphere

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    Wennberg, P. O.; Hanisco, T. F.; Jaegle, L.; Jacob, D. J.; Hintsa, E. J.; Lanzendorf, E. J.; Anderson, J. G.; Gao, R.-S.; Keim, E. R.; Donnelly, S. G.; hide

    1998-01-01

    The concentrations of the hydrogen radicals OH and HO2 in the middle and upper troposphere were measured simultaneously with those of NO, O3, CO, H2O, CH4, non-methane hydrocarbons, and with the ultraviolet and visible radiation field. The data allow a direct examination of the processes that produce O3, in this region of the atmosphere. Comparison of the measured concentrations of OH and HO2 with calculations based on their production from water vapor, ozone, and methane demonstrate that these sources are insufficient to explain the observed radical concentrations in the upper troposphere. The photolysis of carbonyl and peroxide compounds transported to this region from the lower troposphere may provide the source of HO(x) required to sustain the measured abundances of these radical species. The mechanism by which NO affects the production of 03 is also illustrated by the measurements. In the upper tropospheric air masses sampled, the production rate for ozone (determined from the measured concentrations of HO2 and NO) is calculated to be about 1 part per billion by volume each day.This production rate is faster than previously thought and implies that anthropogenic activities that add NO to the upper troposphere, such as biomass burning and aviation, will lead to production of more 03 than expected.

  20. On the impact of aircraft emitted NO{sub x} on upper troposphere photochemistry

    Energy Technology Data Exchange (ETDEWEB)

    Wahner, A; Rohrer, F; Ehhalt, D H [Forschungszentrum Juelich GmbH (Germany). Inst. fuer Atmosphaerische Chemie

    1998-12-31

    The enhanced nitrogen oxide concentrations influence the photochemical production of ozone as well as the steady state concentrations of hydroxyl radicals, OH, in the upper troposphere. That increase is small compared to the impact of NO{sub x} from fossil fuel combustion on boundary layer ozone. A simple quasi 2-D model was used for the latitude band 40 deg - 50 deg N to analyze the reasons for that. The model includes a simplified CH{sub 4} - CO chemistry and the salient sources of upper tropospheric NO{sub x}, namely lightning, stratospheric input, aircraft emissions and fast upward transport of surface emissions. It is shown that the maximum of net O{sub 3} production and OH concentrations occur at much lower NO{sub x} mixing ratios than in the lower troposphere. (author)

  1. On the impact of aircraft emitted NO{sub x} on upper troposphere photochemistry

    Energy Technology Data Exchange (ETDEWEB)

    Wahner, A.; Rohrer, F.; Ehhalt, D.H. [Forschungszentrum Juelich GmbH (Germany). Inst. fuer Atmosphaerische Chemie

    1997-12-31

    The enhanced nitrogen oxide concentrations influence the photochemical production of ozone as well as the steady state concentrations of hydroxyl radicals, OH, in the upper troposphere. That increase is small compared to the impact of NO{sub x} from fossil fuel combustion on boundary layer ozone. A simple quasi 2-D model was used for the latitude band 40 deg - 50 deg N to analyze the reasons for that. The model includes a simplified CH{sub 4} - CO chemistry and the salient sources of upper tropospheric NO{sub x}, namely lightning, stratospheric input, aircraft emissions and fast upward transport of surface emissions. It is shown that the maximum of net O{sub 3} production and OH concentrations occur at much lower NO{sub x} mixing ratios than in the lower troposphere. (author)

  2. How predictable is the northern hemisphere summer upper-tropospheric circulation?

    Energy Technology Data Exchange (ETDEWEB)

    Lee, June-Yi; Wang, Bin [University of Hawaii/IPRC, International Pacific Research Center, Honolulu, HI (United States); Ding, Q. [University of Washington, Department of Earth and Space Sciences and Quaternary Research Center, Seattle, WA (United States); Ha, K.J.; Ahn, J.B. [Pusan National University, Division of Earth Environmental System, Busan (Korea, Republic of); Kumar, A. [NCEP/CPC, Camp Springs, MD (United States); Stern, B. [Princeton University, NOAA/GFDL, Princeton, NJ (United States); Alves, O. [Bureau of Meteorology, Centre for Australia Weather and Climate Research (CAWCR), Melbourne, VIC (Australia)

    2011-09-15

    The retrospective forecast skill of three coupled climate models (NCEP CFS, GFDL CM2.1, and CAWCR POAMA 1.5) and their multi-model ensemble (MME) is evaluated, focusing on the Northern Hemisphere (NH) summer upper-tropospheric circulation along with surface temperature and precipitation for the 25-year period of 1981-2005. The seasonal prediction skill for the NH 200-hPa geopotential height basically comes from the coupled models' ability in predicting the first two empirical orthogonal function (EOF) modes of interannual variability, because the models cannot replicate the residual higher modes. The first two leading EOF modes of the summer 200-hPa circulation account for about 84% (35.4%) of the total variability over the NH tropics (extratropics) and offer a hint of realizable potential predictability. The MME is able to predict both spatial and temporal characteristics of the first EOF mode (EOF1) even at a 5-month lead (January initial condition) with a pattern correlation coefficient (PCC) skill of 0.96 and a temporal correlation coefficient (TCC) skill of 0.62. This long-lead predictability of the EOF1 comes mainly from the prolonged impacts of El Nino-Southern Oscillation (ENSO) as the EOF1 tends to occur during the summer after the mature phase of ENSO. The second EOF mode (EOF2), on the other hand, is related to the developing ENSO and also the interdecadal variability of the sea surface temperature over the North Pacific and North Atlantic Ocean. The MME also captures the EOF2 at a 5-month lead with a PCC skill of 0.87 and a TCC skill of 0.67, but these skills are mainly obtained from the zonally symmetric component of the EOF2, not the prominent wavelike structure, the so-called circumglobal teleconnection (CGT) pattern. In both observation and the 1-month lead MME prediction, the first two leading modes are accompanied by significant rainfall and surface air temperature anomalies in the continental regions of the NH extratropics. The MME

  3. Hydrogen Radicals, Nitrogen Radicals, and the Production of Ozone in the Middle and Upper Troposphere

    Science.gov (United States)

    Bui, T. P.

    1997-01-01

    The concentrations of hydrogen radicals, OH and HO2, in the middle and upper troposphere were measured simultaneously with those of NO, O3,CO, H20, CH4, non-methane hydrocarbons, and with the ultraviolet and visible radiation field.

  4. The role of chemistry in under-predictions of NO2 in the upper troposphere

    Science.gov (United States)

    Henderson, B. H.; Pinder, R. W.; Goliff, W. S.; Stockwell, W. R.; Fahr, A.; Sarwar, G.; Hutzell, W. T.; Mathur, R.; Vizuete, W.; Cohen, R. C.

    2009-12-01

    Global and regional atmospheric models under-predict upper troposphere NO2 compared to satellite and aircraft observations. The upper tropospheric under-prediction of NO2 could be a function of emissions, transport, chemistry or some combination. Previous researchers have linked poor performance in the model to over-prediction of the OH and under-prediction of the HO2 by chemistry (Olson et al. 2006, Bertram et al. 2007). This study isolates upper tropospheric chemistry to evaluate the chemical contribution to NO2 under-predictions and to diagnose OH and HO2 discrepancies. We use a 0-dimensional time dependent model to evaluate seven chemical mechanisms. Because chamber data representing upper tropospheric conditions does not exist, we evaluate the predictions based against an observation-based aging model. Following Bertram et al (2007), we use the NOx:HNO3 ratio to categorize the chemical age of thousands of 10 second average observations between 8 and 10km. Measurements of 10 inorganics and 32 hydrocarbons are translated to model species for each of seven chemical mechanisms. We chose mechanisms ranging from condensed to semi-explicit. The seven mechanisms' design scopes range from urban to global scale. Results include simulations from Model for OZone And Related chemical Tracers (MOZART), Carbon Bond 05 (CB05), State Air Pollution Research Center (SAPRC) 99, SAPRC 07, GEOS-Chem, Regional Atmospheric Chemical Mechanism version 2, and the LEEDS Master Chemical Mechanism. Results from each chemical mechanism are compared to aircraft observations and to those obtained with other chemical mechanisms. Each mechanism is then further evaluated using integrated reaction rate analysis to identify sources of NO2 bias. We find that the largest contributors to the NO2 bias are over-predictions of PAN and HNO3. The formation of PAN is sensitive to the acetone photolysis rate. The conversion of NOx to HNO3 is most sensitive to hydroxyl radical concentrations. Hydroxyl

  5. Reanalysis comparisons of upper tropospheric-lower stratospheric jets and multiple tropopauses

    Science.gov (United States)

    Manney, Gloria L.; Hegglin, Michaela I.; Lawrence, Zachary D.; Wargan, Krzysztof; Millán, Luis F.; Schwartz, Michael J.; Santee, Michelle L.; Lambert, Alyn; Pawson, Steven; Knosp, Brian W.; Fuller, Ryan A.; Daffer, William H.

    2017-09-01

    The representation of upper tropospheric-lower stratospheric (UTLS) jet and tropopause characteristics is compared in five modern high-resolution reanalyses for 1980 through 2014. Climatologies of upper tropospheric jet, subvortex jet (the lowermost part of the stratospheric vortex), and multiple tropopause frequency distributions in MERRA (Modern-Era Retrospective analysis for Research and Applications), ERA-I (ERA-Interim; the European Centre for Medium-Range Weather Forecasts, ECMWF, interim reanalysis), JRA-55 (the Japanese 55-year Reanalysis), and CFSR (the Climate Forecast System Reanalysis) are compared with those in MERRA-2. Differences between alternate products from individual reanalysis systems are assessed; in particular, a comparison of CFSR data on model and pressure levels highlights the importance of vertical grid spacing. Most of the differences in distributions of UTLS jets and multiple tropopauses are consistent with the differences in assimilation model grids and resolution - for example, ERA-I (with coarsest native horizontal resolution) typically shows a significant low bias in upper tropospheric jets with respect to MERRA-2, and JRA-55 (the Japanese 55-year Reanalysis) a more modest one, while CFSR (with finest native horizontal resolution) shows a high bias with respect to MERRA-2 in both upper tropospheric jets and multiple tropopauses. Vertical temperature structure and grid spacing are especially important for multiple tropopause characterizations. Substantial differences between MERRA and MERRA-2 are seen in mid- to high-latitude Southern Hemisphere (SH) winter upper tropospheric jets and multiple tropopauses as well as in the upper tropospheric jets associated with tropical circulations during the solstice seasons; some of the largest differences from the other reanalyses are seen in the same times and places. Very good qualitative agreement among the reanalyses is seen between the large-scale climatological features in UTLS jet and

  6. A comparison of lightning and aircraft sources of NO{sub x} in the upper troposphere

    Energy Technology Data Exchange (ETDEWEB)

    Penner, J E; Walton, J J [Michigan Univ., Ann Arbor, MI (United States). Dept. of Atmospheric, Oceanic and Space Physics; Bergmann, D J; Kinnison, D; Rotman, D [Lawrence Livermore National Lab., CA (United States). Atmospheric Science Div.; Price, C [Tel Aviv Univ. (Israel). Dept. of Geophysics and Planetary Sciences; Prather, M J [California Univ., Irvine, CA (United States). Dept. of Earth System Science; Pickering, K E [Maryland Univ., College Park, MD (United States). Dept. of Meteorology; Baughcum, S L [Boeing Commerial Airplane Group, Seatlle, WA (United States)

    1998-12-31

    Uncertainties in the assessment of the contribution of aircraft to upper tropospheric NO{sub x} arise from uncertainties in model treatment of transport, uncertainties in source strengths, and uncertainties in chemical rates and reactions determining the partitioning between NO{sub x} and NO{sub y}. Two different chemical transport models are used to examine the range of uncertainty in the contribution of aircraft to upper tropospheric NO{sub x} from model representations of transport. Uncertainties caused by uncertainties in the rate of production of NO{sub x} from lightning and uncertainties from the range of background concentrations of HNO{sub 3} are also examined. Uncertainties in the treatment of vertical transport and uncertainties in the source strength from lightning contribute to a large range in model results for background NO{sub x}. (author) 18 refs.

  7. A comparison of lightning and aircraft sources of NO{sub x} in the upper troposphere

    Energy Technology Data Exchange (ETDEWEB)

    Penner, J.E.; Walton, J.J. [Michigan Univ., Ann Arbor, MI (United States). Dept. of Atmospheric, Oceanic and Space Physics; Bergmann, D.J.; Kinnison, D.; Rotman, D. [Lawrence Livermore National Lab., CA (United States). Atmospheric Science Div.; Price, C. [Tel Aviv Univ. (Israel). Dept. of Geophysics and Planetary Sciences; Prather, M.J. [California Univ., Irvine, CA (United States). Dept. of Earth System Science; Pickering, K.E. [Maryland Univ., College Park, MD (United States). Dept. of Meteorology; Baughcum, S.L. [Boeing Commerial Airplane Group, Seatlle, WA (United States)

    1997-12-31

    Uncertainties in the assessment of the contribution of aircraft to upper tropospheric NO{sub x} arise from uncertainties in model treatment of transport, uncertainties in source strengths, and uncertainties in chemical rates and reactions determining the partitioning between NO{sub x} and NO{sub y}. Two different chemical transport models are used to examine the range of uncertainty in the contribution of aircraft to upper tropospheric NO{sub x} from model representations of transport. Uncertainties caused by uncertainties in the rate of production of NO{sub x} from lightning and uncertainties from the range of background concentrations of HNO{sub 3} are also examined. Uncertainties in the treatment of vertical transport and uncertainties in the source strength from lightning contribute to a large range in model results for background NO{sub x}. (author) 18 refs.

  8. Upper tropospheric cloud systems determined from IR Sounders and their influence on the atmosphere

    Science.gov (United States)

    Stubenrauch, Claudia; Protopapadaki, Sofia; Feofilov, Artem; Velasco, Carola Barrientos

    2017-02-01

    Covering about 30% of the Earth, upper tropospheric clouds play a key role in the climate system by modulating the Earth's energy budget and heat transport. Infrared Sounders reliably identify cirrus down to an IR optical depth of 0.1. Recently LMD has built global cloud climate data records from AIRS and IASI observations, covering the periods from 2003-2015 and 2008-2015, respectively. Upper tropospheric clouds often form mesoscale systems. Their organization and properties are being studied by (1) distinguishing cloud regimes within 2° × 2° regions and (2) applying a spatial composite technique on adjacent cloud pressures, which estimates the horizontal extent of the mesoscale cloud systems. Convective core, cirrus anvil and thin cirrus of these systems are then distinguished by their emissivity. Compared to other studies of tropical mesoscale convective systems our data include also the thinner anvil parts, which make out about 30% of the area of tropical mesoscale convective systems. Once the horizontal and vertical structure of these upper tropospheric cloud systems is known, we can estimate their radiative effects in terms of top of atmosphere and surface radiative fluxes and by computing their heating rates.

  9. The zonal structure of tropical O3 and CO as observed by the Tropospheric Emission Spectrometer in November 2004 – Part 2: Impact of surface emissions on O3 and its precursors

    Directory of Open Access Journals (Sweden)

    G. Osterman

    2009-06-01

    Full Text Available The impact of surface emissions on the zonal structure of tropical tropospheric ozone and carbon monoxide is investigated for November 2004 using satellite observations, in-situ measurements, and chemical transport models in conjunction with inverse-estimated surface emissions.Vertical ozone profiles from the Tropospheric Emission Spectrometer (TES and ozone sonde measurements from the Southern Hemisphere Additional Ozonesondes (SHADOZ network show elevated concentrations of ozone over Indonesia and Australia (60–70 ppb in the lower troposphere against the backdrop of the well-known zonal "wave-one" pattern with ozone concentrations of (70–80 ppb centered over the Atlantic . Observational evidence from TES CO vertical profiles and Ozone Monitoring Instrument (OMI NO2 columns point to regional surface emissions as an important contributor to the elevated ozone over Indonesia. This contribution is investigated with the GEOS-Chem chemistry and transport model using surface emission estimates derived from an optimal inverse model, which was constrained by TES and Measurements Of Pollution In The Troposphere (MOPITT CO profiles (Jones et al., 2009. These a posteriori estimates, which were over a factor of 2 greater than climatological emissions, reduced differences between GEOS-Chem and TES ozone observations by 30–40% over Indonesia. The response of the free tropospheric chemical state to the changes in these emissions is investigated for ozone, CO, NOx, and PAN. Model simulations indicate that ozone over Indonesian/Australian is sensitive to regional changes in surface emissions of NOx but relatively insensitive to lightning NOx. Over sub-equatorial Africa and South America, free tropospheric NOx was reduced in response to increased surface emissions potentially muting ozone production.

  10. Surface measurements of upper tropospheric water vapor isotopic composition on the Chajnantor Plateau, Chile

    Science.gov (United States)

    Galewsky, Joseph; Rella, Christopher; Sharp, Zachary; Samuels, Kimberly; Ward, Dylan

    2011-09-01

    Simultaneous, real-time measurements of atmospheric water vapor mixing ratio and isotopic composition (δD and δ18O) were obtained using cavity ringdown spectroscopy on the arid Chajnantor Plateau in the subtropical Chilean Andes (elevation 5080 m or 550 hPa; latitude 23°S) during July and August 2010. The measurements show surface water vapor mixing ratio as low as 215 ppmv, δD values as low as -540‰, and δ18O values as low as -68‰, which are the lowest atmospheric water vapor δ values reported from Earth's surface. The results are consistent with previous measurements from the base of the tropical tropopause layer (TTL) and suggest large-scale subsidence of air masses from the upper troposphere to the Earth's surface. The range of measurements is consistent with condensation under conditions of ice supersaturation and mixing with moister air from the lower troposphere that has been processed through shallow convection. Diagnostics using reanalysis data show that the extreme aridity of the Chajnantor Plateau is controlled by condensation in the upper tropical troposphere.

  11. Influence of isentropic transport on seasonal ozone variations in the lower stratosphere and subtropical upper troposphere

    Science.gov (United States)

    Jing, P.; Cunnold, D. M.; Yang, E.-S.; Wang, H.-J.

    2005-01-01

    The isentropic cross-tropopause ozone transport has been estimated in both hemispheres in 1999 based on the potential vorticity mapping of Stratospheric Aerosol and Gas Experiment 11 ozone measurements and contour advection calculations using the NASA Goddard Space Flight Center Global and Modeling Assimilation Office analysis. The estimated net isentropic stratosphere-to-troposphere ozone flux is approx.118 +/- 61 x 10(exp9)kg/yr globally within the layer between 330 and 370 K in 1999; 60% of it is found in the Northern Hemisphere, and 40% is found in the Southern Hemisphere. The monthly average ozone fluxes are strongest in summer and weakest in winter in both hemispheres. The seasonal variations of ozone in the lower stratosphere (LS) and upper troposphere (UT) have been analyzed using ozonesonde observations from ozonesonde stations in the extratropics and subtropics, respectively. It is shown that observed ozone levels increase in the UT over subtropical ozonesonde stations and decrease in the LS over extratropical stations in late spring/early summer and that the ozone increases in the summertime subtropical UT are unlikely to be explained by photochemical ozone production and diabatic transport alone. We conclude that isentropic transport is a significant contributor to ozone levels in the subtropical upper troposphere, especially in summer.

  12. Upper Troposphere Lower Stratosphere structure during convective systems using GPS radio occultations

    DEFF Research Database (Denmark)

    Biondi, Riccardo

    The deep convective systems play a fundamental role in atmospheric circulation and climate. Thunderstorms and meso-scale convective systems produce fast vertical transport, redistributing water vapor and trace gases and influencing the thermal structure of the upper troposphere and lower...... stratosphere (UTLS) contributing to the troposphere-stratosphere transport and affecting the Earth global circulation and the climate changes. The Global Positioning System (GPS) Radio Occultation (RO) technique enables measurement of atmospheric density structure in any meteorological condition...... to the analysis of tropical storms for the future mission ACES will also be evaluated. Using data from the past and ongoing GPS RO missions we have defined an algorithm to detect the clouds top of the convective systems and their thermal structure. Other satellite and in-situ measurements co-located with GPS ROs...

  13. The Ozone Budget in the Upper Troposphere from Global Modeling Initiative (GMI)Simulations

    Science.gov (United States)

    Rodriquez, J.; Duncan, Bryan N.; Logan, Jennifer A.

    2006-01-01

    Ozone concentrations in the upper troposphere are influenced by in-situ production, long-range tropospheric transport, and influx of stratospheric ozone, as well as by photochemical removal. Since ozone is an important greenhouse gas in this region, it is particularly important to understand how it will respond to changes in anthropogenic emissions and changes in stratospheric ozone fluxes.. This response will be determined by the relative balance of the different production, loss and transport processes. Ozone concentrations calculated by models will differ depending on the adopted meteorological fields, their chemical scheme, anthropogenic emissions, and treatment of the stratospheric influx. We performed simulations using the chemical-transport model from the Global Modeling Initiative (GMI) with meteorological fields from (It)h e NASA Goddard Institute for Space Studies (GISS) general circulation model (GCM), (2) the atmospheric GCM from NASA's Global Modeling and Assimilation Office(GMAO), and (3) assimilated winds from GMAO . These simulations adopt the same chemical mechanism and emissions, and adopt the Synthetic Ozone (SYNOZ) approach for treating the influx of stratospheric ozone -. In addition, we also performed simulations for a coupled troposphere-stratosphere model with a subset of the same winds. Simulations were done for both 4degx5deg and 2degx2.5deg resolution. Model results are being tested through comparison with a suite of atmospheric observations. In this presentation, we diagnose the ozone budget in the upper troposphere utilizing the suite of GMI simulations, to address the sensitivity of this budget to: a) the different meteorological fields used; b) the adoption of the SYNOZ boundary condition versus inclusion of a full stratosphere; c) model horizontal resolution. Model results are compared to observations to determine biases in particular simulations; by examining these comparisons in conjunction with the derived budgets, we may pinpoint

  14. Seasonality of Peroxyacetyl nitrate (PAN in the upper troposphere and lower stratosphere using the MIPAS-E instrument

    Directory of Open Access Journals (Sweden)

    D. P. Moore

    2010-07-01

    Full Text Available The Michelson Interferometer for Passive Atmospheric Sounding onboard ENVISAT (MIPAS–E offers the opportunity to detect and spectrally resolve many atmospheric minor constituents affecting atmospheric chemistry. In this paper, we retrieve global, seasonal PAN volume mixing ratio (vmr data from MIPAS-E measurements made in January, March, August and October 2003 and present results from this scheme between approximately 300 and 150 hPa. The total error on a single PAN retrieval is better than 20% outside the tropics and better than 50% in the tropics where uncertainties in water vapor dominate the total error budget. We observe clear differences in the seasonal cycle of PAN in our data, linked closely to biomass burning regions and growing seasons. Highest Northern Hemisphere mid-latitude PAN vmrs were observed in August (300–600 pptv on average compared with the January and October data (less than 250 pptv on average. In the March 2003 data we observe highest PAN vmrs in the tropics with evidence of vmrs between 600 and 1000 pptv over Eastern Asia and over the Central Pacific at 333 hPa. The vertical distribution of PAN as a function of latitude (i.e. the zonal mean highlights the strong inter-annual variability of PAN in the upper troposphere and lower stratosphere (UTLS, most pronounced poleward of 40° N (up to 400 pptv over the year. The variability of PAN in the tropical UTLS is also significant and we derive a variability of up to 250 pptv in the averages between January and October 2003. These results represent the first seasonal observations of PAN in the UTLS.

  15. Upper-tropospheric CO and O3 budget during the Asian summer monsoon

    Directory of Open Access Journals (Sweden)

    B. Barret

    2016-07-01

    Full Text Available During the Asian summer monsoon, the circulation in the upper troposphere/lower stratosphere (UTLS is dominated by the Asian monsoon anticyclone (AMA. Pollutants convectively uplifted to the upper troposphere are trapped within this anticyclonic circulation that extends from the Pacific Ocean to the Eastern Mediterranean basin. Among the uplifted pollutants are ozone (O3 and its precursors, such as carbon monoxide (CO and nitrogen oxides (NOx. Many studies based on global modeling and satellite data have documented the source regions and transport pathways of primary pollutants (CO, HCN into the AMA. Here, we aim to quantify the O3 budget by taking into consideration anthropogenic and natural sources. We first use CO and O3 data from the MetOp-A/IASI sensor to document their tropospheric distributions over Asia, taking advantage of the useful information they provide on the vertical dimension. These satellite data are used together with MOZAIC tropospheric profiles recorded in India to validate the distributions simulated by the global GEOS-Chem chemistry transport model. Over the Asian region, UTLS monthly CO and O3 distributions from IASI and GEOS-Chem display the same large-scale features. UTLS CO columns from GEOS-Chem are in agreement with IASI, with a low bias of 11 ± 9 % and a correlation coefficient of 0.70. For O3, the model underestimates IASI UTLS columns over Asia by 14 ± 26 % but the correlation between both is high (0.94. GEOS-Chem is further used to quantify the CO and O3 budget through sensitivity simulations. For CO, these simulations confirm that South Asian anthropogenic emissions have a more important impact on enhanced concentrations within the AMA (∼  25 ppbv than East Asian emissions (∼  10 ppbv. The correlation between enhanced emissions over the Indo-Gangetic Plain and monsoon deep convection is responsible for this larger impact. Consistently, South Asian anthropogenic NOx emissions also

  16. Observations of peroxyacetyl nitrate (PAN) in the upper troposphere by the Atmospheric Chemistry Experiment-Fourier Transform Spectrometer (ACE-FTS)

    Science.gov (United States)

    Tereszchuk, K. A.; Moore, D. P.; Harrison, J. J.; Boone, C. D.; Park, M.; Remedios, J. J.; Randel, W. J.; Bernath, P. F.

    2013-06-01

    Peroxyacetyl nitrate (CH3CO·O2NO2, abbreviated as PAN) is a trace molecular species present in the troposphere and lower stratosphere due primarily to pollution from fuel combustion and the pyrogenic outflows from biomass burning. In the lower troposphere, PAN has a relatively short lifetime and is principally destroyed within a few hours through thermolysis, but it can act as a reservoir and carrier of NOx in the colder temperatures of the upper troposphere, where UV photolysis becomes the dominant loss mechanism. Pyroconvective updrafts from large biomass burning events can inject PAN into the upper troposphere and lower stratosphere (UTLS), providing a means for the long-range transport of NOx. Given the extended lifetimes at these higher altitudes, PAN is readily detectable via satellite remote sensing. A new PAN data product is now available for the Atmospheric Chemistry Experiment Fourier Transform Spectrometer (ACE-FTS) version 3.0 data set. We report observations of PAN in boreal biomass burning plumes recorded during the BORTAS (quantifying the impact of BOReal forest fires on Tropospheric oxidants over the Atlantic using Aircraft and Satellites) campaign (12 July to 3 August 2011). The retrieval method employed by incorporating laboratory-recorded absorption cross sections into version 3.0 of the ACE-FTS forward model and retrieval software is described in full detail. The estimated detection limit for ACE-FTS PAN is 5 pptv, and the total systematic error contribution to the ACE-FTS PAN retrieval is ~ 16%. The retrieved volume mixing ratio (VMR) profiles are compared to coincident measurements made by the Michelson Interferometer for Passive Atmospheric Sounding (MIPAS) instrument on the European Space Agency (ESA) Environmental Satellite (ENVISAT). The MIPAS measurements demonstrated good agreement with the ACE-FTS VMR profiles for PAN, where the measured VMR values are well within the associated measurement errors for both instruments and comparative

  17. First detection of ammonia (NH3 in the Asian summer monsoon upper troposphere

    Directory of Open Access Journals (Sweden)

    M. Höpfner

    2016-11-01

    Full Text Available Ammonia (NH3 has been detected in the upper troposphere by the analysis of averaged MIPAS (Michelson Interferometer for Passive Atmospheric Sounding infrared limb-emission spectra. We have found enhanced amounts of NH3 within the region of the Asian summer monsoon at 12–15 km altitude. Three-monthly, 10° longitude  ×  10° latitude average profiles reaching maximum mixing ratios of around 30 pptv in this altitude range have been retrieved, with a vertical resolution of 3–8 km and estimated errors of about 5 pptv. These observations show that loss processes during transport from the boundary layer to the upper troposphere within the Asian monsoon do not deplete the air entirely of NH3. Thus, ammonia might contribute to the so-called Asian tropopause aerosol layer by the formation of ammonium aerosol particles. On a global scale, outside the monsoon area and during different seasons, we could not detect enhanced values of NH3 above the actual detection limit of about 3–5 pptv. This upper bound helps to constrain global model simulations.

  18. Generation of layering in the upper arctic troposphere away from the jet stream

    Directory of Open Access Journals (Sweden)

    A. Karpetchko

    Full Text Available Ozone sounding databases for two stations, So-dankylä (67° N, 27° E and Ny-Ålesund (79° N, 12° E were used in order to investigate the generation of layering in the upper and middle troposphere of the Arctic. We concentrated on dry, ozone-rich and stable layers observed below the thermal tropopause under light wind conditions. This condition ensures that the observed layer is not a tropopause fold, a well-known phenomenon that develops within frontal zones near the jet stream. Selection criteria for ozone, humidity and stability anomalies of the tropopause fold detection algorithm were used here to pick out for detailed studies the most pronounced examples of laminae. For all these cases the meteorological situations were investigated in order to establish the origin of the observed layers. We found that layers could be classified into two groups. Laminae of the first group were observed equatorward of the jet stream and those of a second group were observed poleward of the jet. The meteorological situation for the first group resembles that for equatorward stratospheric streamer propagation. It was found that this group accounts for only a small fraction of the layers observed at Sodankylä and for none of those observed at Ny-Ålesund during the period investigated. A large case-to-case variability in the synoptic situation was observed for the second group of laminae, which were detected northward of the jet stream. Nevertheless, in about half of the cases, streamers of tropospheric air were found in the vicinity of the stations on the isentropic surfaces just above the detected stratospheric layers. Back trajectory analyses showed that these layers originated in the vicinity of the polar jet stream. We suppose that laminae-like structures in the troposphere were caused, in both groups, by equatorward (poleward advection of the stratospheric (tropospheric air, together with differential vertical shear. Forward-trajectory calculations

  19. Generation of layering in the upper arctic troposphere away from the jet stream

    Directory of Open Access Journals (Sweden)

    A. Karpetchko

    2003-07-01

    Full Text Available Ozone sounding databases for two stations, So-dankylä (67° N, 27° E and Ny-Ålesund (79° N, 12° E were used in order to investigate the generation of layering in the upper and middle troposphere of the Arctic. We concentrated on dry, ozone-rich and stable layers observed below the thermal tropopause under light wind conditions. This condition ensures that the observed layer is not a tropopause fold, a well-known phenomenon that develops within frontal zones near the jet stream. Selection criteria for ozone, humidity and stability anomalies of the tropopause fold detection algorithm were used here to pick out for detailed studies the most pronounced examples of laminae. For all these cases the meteorological situations were investigated in order to establish the origin of the observed layers. We found that layers could be classified into two groups. Laminae of the first group were observed equatorward of the jet stream and those of a second group were observed poleward of the jet. The meteorological situation for the first group resembles that for equatorward stratospheric streamer propagation. It was found that this group accounts for only a small fraction of the layers observed at Sodankylä and for none of those observed at Ny-Ålesund during the period investigated. A large case-to-case variability in the synoptic situation was observed for the second group of laminae, which were detected northward of the jet stream. Nevertheless, in about half of the cases, streamers of tropospheric air were found in the vicinity of the stations on the isentropic surfaces just above the detected stratospheric layers. Back trajectory analyses showed that these layers originated in the vicinity of the polar jet stream. We suppose that laminae-like structures in the troposphere were caused, in both groups, by equatorward (poleward advection of the stratospheric (tropospheric air, together with differential vertical shear. Forward-trajectory calculations

  20. Commentary on using equivalent latitude in the upper troposphere and lower stratosphere

    Directory of Open Access Journals (Sweden)

    L. L. Pan

    2012-10-01

    Full Text Available We discuss the use of potential vorticity (PV based equivalent latitude (EqLat and potential temperature (θ coordinates in the upper troposphere and lower stratosphere (UTLS for chemical transport studies. The main objective is to provide a cautionary note on using EqLat-θ coordinates for aggregating chemical tracers in the UTLS. Several examples are used to show 3-D distributions of EqLat together with chemical constituents for a range of θ. We show that the use of PV-θ coordinates may not be suitable for several reasons when tropospheric processes are an important part of a study. Due to the different static stability structures between the stratosphere and troposphere, the use of θ as a vertical coordinate does not provide equal representations of the UT and LS. Since the θ surfaces in the troposphere often intersect the surface of the Earth, the θ variable does not work well distinguishing the UT from the boundary layer when used globally as a vertical coordinate. We further discuss the duality of PV/EqLat as a tracer versus as a coordinate variable. Using an example, we show that while PV/EqLat serves well as a transport tracer in the UTLS region, it may conceal the chemical structure associated with wave breaking when used as a coordinate to average chemical tracers. Overall, when choosing these coordinates, considerations need to be made not only based on the time scale of PV being a conservative tracer, but also the specific research questions to be addressed.

  1. submitter Technical Note: Using DEG-CPCs at upper tropospheric temperatures

    CERN Document Server

    Wimmer, D; Nieminen, T; Duplissy, J; Ehrhart, S; Almeida, J; Rondo, L; Franchin, A; Kreissl, F; Bianchi, F; Manninen, H E; Kulmala, M; Curtius, J; Petäjä, T

    2015-01-01

    Over the last few years, several condensation particle counters (CPCs) capable of measuring in the sub-3 nm size range have been developed. Here we study the performance of CPCs based on diethylene glycol (DEG) at different temperatures during Cosmics Leaving OUtdoor Droplets (CLOUD) measurements at CERN. The data shown here are the first set of verification measurements for sub-3 nm CPCs under upper tropospheric temperatures using atmospherically relevant aerosol particles. To put the results in perspective we calibrated the DEG-CPC at room temperature, resulting in a cut-off diameter of 1.4 nm. All diameters refer to mobility equivalent diameters in this paper. At upper tropospheric temperatures ranging from 246.15 K to 207.15 K, we found cut-off sizes relative to a particle size magnifier in the range of 2.5 to 2.8 nm. Due to low number concentration after size classification, the cut-off diameters have a high uncertainty (±0.3 nm) associated with them. Operating two laminar flow DEG-CPCs with different c...

  2. Evidence of a 50-year increase in tropospheric ozone in Upper Bavaria

    Directory of Open Access Journals (Sweden)

    M. Schmidt

    Full Text Available In a series of ozone-sonde soundings at the Hohenpeißenberg observatory, starting in 1967, the most striking features are increases of sim2.2% per year in all tropospheric heights up to 8 km during the past 24 years. These facts have recently been published and discussed by several authors. In this paper, we present some evidence for the increase of tropospheric ozone concentrations during the past 50 years 1940-1990 in the territory of the northern edge of the Bavarian Alps, including the Hohenpeißenberg data. In December 1940 and August 1942, probably the first exact wet-chemical vertical soundings of ozone up to 9 km height were made by an aircraft in the region mentioned. These results were published in the earlier literature. We have converted the results of the flights on 4 days in December 1940 and on 6 days in August 1942 to modern units and have compared them with the Hohenpeißenberg ozone-sonde data of the December and August months. We also compared the data at the ground with the August results of Paris-Montsouris 1886-1898. Our results show an increase of ozone concentration at all tropospheric heights in Upper Bavaria during the past 50 years, compared with the Montsouris data in August during the past 105 years. In the recently published papers, the increases since 1967 were approximated linearly.Our results, extended to the past, show non-linear trends, with steeper increases since 1975-1979. Possible reasons for these findings are discussed. Quite recently (in case of the December months since 1986/87, the August months since 1990, the ozone mixing ratios at and above Hohenpeißenberg seem to have decreased.

  3. Evidence of a 50-year increase in tropospheric ozone in Upper Bavaria

    Directory of Open Access Journals (Sweden)

    M. Schmidt

    1994-12-01

    Full Text Available In a series of ozone-sonde soundings at the Hohenpeißenberg observatory, starting in 1967, the most striking features are increases of \\sim2.2% per year in all tropospheric heights up to 8 km during the past 24 years. These facts have recently been published and discussed by several authors. In this paper, we present some evidence for the increase of tropospheric ozone concentrations during the past 50 years 1940-1990 in the territory of the northern edge of the Bavarian Alps, including the Hohenpeißenberg data. In December 1940 and August 1942, probably the first exact wet-chemical vertical soundings of ozone up to 9 km height were made by an aircraft in the region mentioned. These results were published in the earlier literature. We have converted the results of the flights on 4 days in December 1940 and on 6 days in August 1942 to modern units and have compared them with the Hohenpeißenberg ozone-sonde data of the December and August months. We also compared the data at the ground with the August results of Paris-Montsouris 1886-1898. Our results show an increase of ozone concentration at all tropospheric heights in Upper Bavaria during the past 50 years, compared with the Montsouris data in August during the past 105 years. In the recently published papers, the increases since 1967 were approximated linearly.Our results, extended to the past, show non-linear trends, with steeper increases since 1975-1979. Possible reasons for these findings are discussed. Quite recently (in case of the December months since 1986/87, the August months since 1990, the ozone mixing ratios at and above Hohenpeißenberg seem to have decreased.

  4. CARIBIC observations of gaseous mercury in the upper troposphere and lower stratosphere

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    Slemr F.

    2013-04-01

    Full Text Available A unique set of gaseous mercury measurements in the upper troposphere and lower stratosphere (UT/LS has been obtained during the monthly CARIBIC (www.caribic-atmospheric.com flights since May 2005. The passenger Airbus 340-600 of Lufthansa covered routes to the Far East, North America, India, and the southern hemisphere. The accompanying measurements of CO, O3, NOy, H2O, aerosols, halocarbons, hydrocarbons, greenhouse gases, and several other parameters as well as backward trajectories enable a detailed analysis of these measurements. Speciation tests have shown that the CARIBIC measurements represent a good approximation of total gaseous mercury (TGM concentrations. Above the tropopause TGM always decrease with increasing potential vorticity (PV and O3 which implies its conversion to particle bound mercury. The observation of the lowest TGM concentrations at the highest particle concentrations in the stratosphere provides further evidence for such conversion. We will show how a seasonally dependent conversion rate could be derived using concomitantly measured SF6 mixing ratios as a timer. Tropospheric mercury data suggest the existence of a decreasing trend in the northern hemisphere whose size is comparable with the trend derived from long-term measurements by ship cruises, at Cape Point (South Africa and Mace Head (Ireland.

  5. Large differences in reanalyses of diabatic heating in the tropical upper troposphere and lower stratosphere

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    J. S. Wright

    2013-09-01

    Full Text Available We present the time mean heat budgets of the tropical upper troposphere (UT and lower stratosphere (LS as simulated by five reanalysis models: the Modern-Era Retrospective Analysis for Research and Applications (MERRA, European Reanalysis (ERA-Interim, Climate Forecast System Reanalysis (CFSR, Japanese 25-yr Reanalysis and Japan Meteorological Agency Climate Data Assimilation System (JRA-25/JCDAS, and National Centers for Environmental Prediction/National Center for Atmospheric Research (NCEP/NCAR Reanalysis 1. The simulated diabatic heat budget in the tropical UTLS differs significantly from model to model, with substantial implications for representations of transport and mixing. Large differences are apparent both in the net heat budget and in all comparable individual components, including latent heating, heating due to radiative transfer, and heating due to parameterised vertical mixing. We describe and discuss the most pronounced differences. Discrepancies in latent heating reflect continuing difficulties in representing moist convection in models. Although these discrepancies may be expected, their magnitude is still disturbing. We pay particular attention to discrepancies in radiative heating (which may be surprising given the strength of observational constraints on temperature and tropospheric water vapour and discrepancies in heating due to turbulent mixing (which have received comparatively little attention. The largest differences in radiative heating in the tropical UTLS are attributable to differences in cloud radiative heating, but important systematic differences are present even in the absence of clouds. Local maxima in heating and cooling due to parameterised turbulent mixing occur in the vicinity of the tropical tropopause.

  6. Large differences in reanalyses of diabatic heating in the tropical upper troposphere and lower stratosphere

    Science.gov (United States)

    Wright, J. S.; Fueglistaler, S.

    2013-09-01

    We present the time mean heat budgets of the tropical upper troposphere (UT) and lower stratosphere (LS) as simulated by five reanalysis models: the Modern-Era Retrospective Analysis for Research and Applications (MERRA), European Reanalysis (ERA-Interim), Climate Forecast System Reanalysis (CFSR), Japanese 25-yr Reanalysis and Japan Meteorological Agency Climate Data Assimilation System (JRA-25/JCDAS), and National Centers for Environmental Prediction/National Center for Atmospheric Research (NCEP/NCAR) Reanalysis 1. The simulated diabatic heat budget in the tropical UTLS differs significantly from model to model, with substantial implications for representations of transport and mixing. Large differences are apparent both in the net heat budget and in all comparable individual components, including latent heating, heating due to radiative transfer, and heating due to parameterised vertical mixing. We describe and discuss the most pronounced differences. Discrepancies in latent heating reflect continuing difficulties in representing moist convection in models. Although these discrepancies may be expected, their magnitude is still disturbing. We pay particular attention to discrepancies in radiative heating (which may be surprising given the strength of observational constraints on temperature and tropospheric water vapour) and discrepancies in heating due to turbulent mixing (which have received comparatively little attention). The largest differences in radiative heating in the tropical UTLS are attributable to differences in cloud radiative heating, but important systematic differences are present even in the absence of clouds. Local maxima in heating and cooling due to parameterised turbulent mixing occur in the vicinity of the tropical tropopause.

  7. Top-of-atmosphere radiative forcing affected by brown carbon in the upper troposphere

    Science.gov (United States)

    Zhang, Yuzhong; Forrister, Haviland; Liu, Jiumeng; Dibb, Jack; Anderson, Bruce; Schwarz, Joshua P.; Perring, Anne E.; Jimenez, Jose L.; Campuzano-Jost, Pedro; Wang, Yuhang; Nenes, Athanasios; Weber, Rodney J.

    2017-07-01

    Carbonaceous aerosols affect the global radiative balance by absorbing and scattering radiation, which leads to warming or cooling of the atmosphere, respectively. Black carbon is the main light-absorbing component. A portion of the organic aerosol known as brown carbon also absorbs light. The climate sensitivity to absorbing aerosols rapidly increases with altitude, but brown carbon measurements are limited in the upper troposphere. Here we present aircraft observations of vertical aerosol distributions over the continental United States in May and June 2012 to show that light-absorbing brown carbon is prevalent in the troposphere, and absorbs more short-wavelength radiation than black carbon at altitudes between 5 and 12 km. We find that brown carbon is transported to these altitudes by deep convection, and that in-cloud heterogeneous processing may produce brown carbon. Radiative transfer calculations suggest that brown carbon accounts for about 24% of combined black and brown carbon warming effect at the tropopause. Roughly two-thirds of the estimated brown carbon forcing occurs above 5 km, although most brown carbon is found below 5 km. The highest radiative absorption occurred during an event that ingested a wildfire plume. We conclude that high-altitude brown carbon from biomass burning is an unappreciated component of climate forcing.

  8. Multi-station synthesis of early twentieth century surface atmospheric electricity measurements for upper tropospheric properties

    Directory of Open Access Journals (Sweden)

    R. G. Harrison

    2007-07-01

    Full Text Available The vertical columnar current density in the global atmospheric electrical circuit depends on the local columnar resistance. A simple model for the columnar resistance is suggested, which separates the local boundary layer component from the upper troposphere cosmic ray component, and calculates the boundary layer component from a surface measurement of air conductivity. This theory is shown to provide reasonable agreement with observations. One application of the simple columnar model theory is to provide a basis for the synthesis of surface atmospheric electrical measurements made simultaneously at several European sites. Assuming the ionospheric potential to be common above all the sites, the theoretical air-earth current density present in the absence of a boundary layer columnar resistance can be found by extrapolation. This is denoted the free troposphere limit air-earth current density, J0. Using early surface data from 1909 when no ionospheric potential data are available for corroboration, J0 is found to be ~6 pA m−2, although this is subject to uncertainties in the data and limitations in the theory. Later (1966–1971 European balloon and surface data give J0=2.4 pA m−2.

  9. Quasi-biweekly oscillations of the South Asian monsoon and its co-evolution in the upper and lower troposphere

    Science.gov (United States)

    Ortega, Sebastián; Webster, Peter J.; Toma, Violeta; Chang, Hai-Ru

    2017-11-01

    The Upper Tropospheric Quasi-Biweekly Oscillation (UQBW) of the South Asian monsoon is studied using the potential vorticity field on the 370 K isentrope. The UQBW is shown to be a common occurrence in the upper troposphere during the monsoon, and its typical evolution is described. We suggest that the UQBW is a phenomenon of both the middle and tropical latitudes, owing its existence to the presence of the planetary-scale upper-tropospheric monsoon anticyclone. The UQBW is first identified as Rossby waves originating in the northern flank of the monsoon anticyclone. These Rossby waves break when reaching the Pacific Ocean, and their associated cyclonic PV anomalies move southward to the east of Asia and then westward across the Indian Ocean and Africa advected by the monsoon anticyclone. A strong correlation, or co-evolution, between the UQBW and quasi-biweekly oscillations in the lower troposphere (QBW) is also found. In particular, analysis of vertically-integrated horizontal moisture transport, 850 hPa geopotential, and outgoing long-wave radiation show that the UQBW is usually observed at the same time as, and co-evolves with, the lower tropospheric QBW over South Asia. We discuss the nature of the UQBW, and its possible physical link with the QBW.

  10. Oxalic acid as a heterogeneous ice nucleus in the upper troposphere and its indirect aerosol effect

    Directory of Open Access Journals (Sweden)

    B. Zobrist

    2006-01-01

    Full Text Available Heterogeneous ice freezing points of aqueous solutions containing various immersed solid dicarboxylic acids (oxalic, adipic, succinic, phthalic and fumaric have been measured with a differential scanning calorimeter. The results show that only the dihydrate of oxalic acid (OAD acts as a heterogeneous ice nucleus, with an increase in freezing temperature between 2 and 5 K depending on solution composition. In several field campaigns, oxalic acid enriched particles have been detected in the upper troposphere with single particle aerosol mass spectrometry. Simulations with a microphysical box model indicate that the presence of OAD may reduce the ice particle number density in cirrus clouds by up to ~50% when compared to exclusively homogeneous cirrus formation without OAD. Using the ECHAM4 climate model we estimate the global net radiative effect caused by this heterogeneous freezing to result in a cooling as high as −0.3 Wm−2.

  11. Global distribution of upper tropospheric formic acid from the ACE-FTS

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    G. González Abad

    2009-10-01

    Full Text Available We present the first near global upper tropospheric distribution of formic acid (HCOOH observed from space using solar occultation measurements from the Fourier transform spectrometer (FTS on board the Atmospheric Chemistry Experiment (ACE satellite. Using a new set of spectroscopic line parameters recently published for formic acid by Vander Auwera et al. (2007 and Perrin and Vander Auwera (2007, we have retrieved the concentrations of HCOOH between 5 km and the tropopause for ACE-FTS observations from February 2004 to September 2007. We observe a significant seasonal dependence for the HCOOH concentrations related to vegetation growth and biomass burning. We estimate an emission ratio of 0.0051±0.0015 for HCOOH relative to CO for tropical South American fires using a selected set of data for September 2004. Results from the balloon-borne MkIV Fourier transform spectrometer are also presented and compared with the ACE measurements.

  12. The Origins of Air Parcels Uplifted in a Two Dimensional Gravity Wave in the Tropical Upper Troposphere During the NASA Stratosphere Troposphere Exchange Project (STEP)

    Science.gov (United States)

    Selkirk, Henry B.; Pfister, Leonhard; Chan, K. Roland; Kritz, Mark; Kelly, Ken

    1989-01-01

    During January and February 1987, as part of the Stratosphere-Troposphere Exchange Project, the NASA ER-2 made 11 flights from Darwin, Australia to investigate dehydration mechanisms in the vicinity of the tropical tropopause. After the monsoon onset in the second week of January, steady easterly flow of 15-25 ms (exp -1) was established in the upper troposphere and lower stratosphere over northern Australia and adjacent seas. Penetrating into this regime were elements of the monsoon convection such as overshooting convective turrets and extensive anvils including cyclone cloud shields. In cases of the latter, the resulting flow obstructions tended to produce mesoscale gravity waves. In several instances the ER- 2 meteorological and trace constituent measurements provide a detailed description of the structure of these gravity waves. Among these was STEP Flight 6, 22-23 January. It is of particular interest to STEP because of the close proximity of ice-laden and dehydrated air on the same isentropic surfaces. Convective events inject large amounts of ice into the upper troposphere and lower stratosphere which may not be completely removed by local precipitation processes. In the present instance, a gravity wave for removed from the source region appears to induce relativity rapid upward motion in the ice-laden air and subsequent dessication. Potential mechanisms for such a localized removal process are under investigation.

  13. EFFECTS OF NON-METHANE HYDROCARBONS ON LOWER STRATOSPHERIC AND UPPER TROPOSPHERIC 2-D ZONAL AVERAGE MODEL CLIMATOLOGY. (R826384)

    Science.gov (United States)

    The perspectives, information and conclusions conveyed in research project abstracts, progress reports, final reports, journal abstracts and journal publications convey the viewpoints of the principal investigator and may not represent the views and policies of ORD and EPA. Concl...

  14. On the Climate Impacts of Upper Tropospheric and Lower Stratospheric Ozone

    Science.gov (United States)

    Xia, Yan; Huang, Yi; Hu, Yongyun

    2018-01-01

    The global warming simulations of the general circulation models (GCMs) are generally performed with different ozone prescriptions. We find that the differences in ozone distribution, especially in the upper tropospheric and lower stratospheric (UTLS) region, account for important model discrepancies shown in the ozone-only historical experiment of the Coupled Model Intercomparison Project Phase 5 (CMIP5). These discrepancies include global high cloud fraction, stratospheric temperature, and stratospheric water vapor. Through a set of experiments conducted by an atmospheric GCM with contrasting UTLS ozone prescriptions, we verify that UTLS ozone not only directly radiatively heats the UTLS region and cools the upper parts of the stratosphere but also strongly influences the high clouds due to its impact on relative humidity and static stability in the UTLS region and the stratospheric water vapor due to its impact on the tropical tropopause temperature. These consequences strongly affect the global mean effective radiative forcing of ozone, as noted in previous studies. Our findings suggest that special attention should be paid to the UTLS ozone when evaluating the climate effects of ozone depletion in the 20th century and recovery in the 21st century. UTLS ozone difference may also be important for understanding the intermodel discrepancy in the climate projections of the CMIP6 GCMs in which either prescribed or interactive ozone is used.

  15. Particulate sulfur in the upper troposphere and lowermost stratosphere – sources and climate forcing

    Directory of Open Access Journals (Sweden)

    B. G. Martinsson

    2017-09-01

    Full Text Available This study is based on fine-mode aerosol samples collected in the upper troposphere (UT and the lowermost stratosphere (LMS of the Northern Hemisphere extratropics during monthly intercontinental flights at 8.8–12 km altitude of the IAGOS-CARIBIC platform in the time period 1999–2014. The samples were analyzed for a large number of chemical elements using the accelerator-based methods PIXE (particle-induced X-ray emission and PESA (particle elastic scattering analysis. Here the particulate sulfur concentrations, obtained by PIXE analysis, are investigated. In addition, the satellite-borne lidar aboard CALIPSO is used to study the stratospheric aerosol load. A steep gradient in particulate sulfur concentration extends several kilometers into the LMS, as a result of increasing dilution towards the tropopause of stratospheric, particulate sulfur-rich air. The stratospheric air is diluted with tropospheric air, forming the extratropical transition layer (ExTL. Observed concentrations are related to the distance to the dynamical tropopause. A linear regression methodology handled seasonal variation and impact from volcanism. This was used to convert each data point into stand-alone estimates of a concentration profile and column concentration of particulate sulfur in a 3 km altitude band above the tropopause. We find distinct responses to volcanic eruptions, and that this layer in the LMS has a significant contribution to the stratospheric aerosol optical depth and thus to its radiative forcing. Further, the origin of UT particulate sulfur shows strong seasonal variation. We find that tropospheric sources dominate during the fall as a result of downward transport of the Asian tropopause aerosol layer (ATAL formed in the Asian monsoon, whereas transport down from the Junge layer is the main source of UT particulate sulfur in the first half of the year. In this latter part of the year, the stratosphere is the clearly dominating source of

  16. On the origin of subvisible cirrus clouds in the tropical upper troposphere

    Directory of Open Access Journals (Sweden)

    M. Reverdy

    2012-12-01

    Full Text Available Spaceborne lidar observations have recently revealed a previously undetected significant population of Subvisible Cirrus (SVC. We show them to be colder than −74 °, with an optical depth below 0.0015 on average. The formation and persistence over time of this new cloud population could be related to several atmospheric phenomena. In this paper, we investigate if these clouds follow the same formation mechanisms as the general tropical cirrus population (including convection and in-situ ice nucleation, or if specific nucleation sites and trace species play a role in their formation. The importance of three scenarios in the formation of the global SVC population is investigated through different approaches that include comparisons with data imaging from several spaceborne instruments and back-trajectories that document the history and behavior of air masses leading to the point in time and space where subvisible cirrus were detected. In order to simplify the study of their formation, we singled out SVC with coherent temperature histories (mean variance lower than 4 K according to back-trajectories along 5, 10 or 15 days (respectively 58, 25 and 11% of SVC. Our results suggest that external processes, including local increases in liquid and hygroscopic aerosol concentration (either through biomass burning or volcanic injection forming sulfate-based aerosols in the troposphere or the stratosphere have very limited short-term or mid-term impact on the SVC population. On the other hand, we find that ~20% of air masses leading to SVC formation interacted with convective activity 5 days before they led to cloud formation and detection, a number that climbs to 60% over 15 days. SVC formation appears especially linked to convection over Africa and Central America, more so during JJA than DJF. These results support the view that the SVC population observed by CALIOP is an extension of the general upper tropospheric ice clouds population with its extreme

  17. Met UM Upper-tropospheric summer jet teleconnections: A model assessment

    Science.gov (United States)

    Joao Carvalho, Maria; Rodriguez, Jose; Milton, Sean

    2017-04-01

    The upper tropospheric jet stream has been documented to act as a waveguide (Hoskins and Ambrizzi, 1993) and supporting quasi-stationary Rossby waves (Schubert et al. 2011). These have been associated with remote effects in surface level weather such as rainfall anomalies in the East Asian Summer Monsoon as well as extreme temperature events. The goal of this work was to analyse the intraseasonal to interannual upper level boreal summer jet variability and its coupling with low level atmospheric dynamics within the Met Office Unified Model using climate runs. Using the Wallace and Gutzler (1981) proposed approach to find teleconnection patterns on the 200 hPa level wind, lead-lag correlation and Empirical Orthogonal Function analysis on the upper-level jet and relating the results with surface weather variables as well as dynamical variables, it was found that the model presents too strong jet variability, particularly in the tropical region and. In addition, the model presents high teleconnectivity hotspots with higher importance in areas such as the Mediterranean and Caspian Sea which are important source areas for Rossby Waves. Further to this, the model was found to produce an area of teleconnectivity between the tropical Atlantic and western Africa which is not observed in the reanalysis but coexists with long lasting precipitation biases. As comparison for the model results, ERA-Interim circulation and wind data and the TRMM precipitation dataset were used. In order to assess the relative importance of relevant model parameters in the biases and process errors, work is currently underway using perturbed model parameter ensembles.

  18. Aerosol characteristics and particle production in the upper troposphere over the Amazon Basin

    Science.gov (United States)

    Andreae, Meinrat O.; Afchine, Armin; Albrecht, Rachel; Amorim Holanda, Bruna; Artaxo, Paulo; Barbosa, Henrique M. J.; Borrmann, Stephan; Cecchini, Micael A.; Costa, Anja; Dollner, Maximilian; Fütterer, Daniel; Järvinen, Emma; Jurkat, Tina; Klimach, Thomas; Konemann, Tobias; Knote, Christoph; Krämer, Martina; Krisna, Trismono; Machado, Luiz A. T.; Mertes, Stephan; Minikin, Andreas; Pöhlker, Christopher; Pöhlker, Mira L.; Pöschl, Ulrich; Rosenfeld, Daniel; Sauer, Daniel; Schlager, Hans; Schnaiter, Martin; Schneider, Johannes; Schulz, Christiane; Spanu, Antonio; Sperling, Vinicius B.; Voigt, Christiane; Walser, Adrian; Wang, Jian; Weinzierl, Bernadett; Wendisch, Manfred; Ziereis, Helmut

    2018-01-01

    Airborne observations over the Amazon Basin showed high aerosol particle concentrations in the upper troposphere (UT) between 8 and 15 km altitude, with number densities (normalized to standard temperature and pressure) often exceeding those in the planetary boundary layer (PBL) by 1 or 2 orders of magnitude. The measurements were made during the German-Brazilian cooperative aircraft campaign ACRIDICON-CHUVA, where ACRIDICON stands for Aerosol, Cloud, Precipitation, and Radiation Interactions and Dynamics of Convective Cloud Systems and CHUVA is the acronym for Cloud Processes of the Main Precipitation Systems in Brazil: A Contribution to Cloud Resolving Modeling and to the GPM (global precipitation measurement), on the German High Altitude and Long Range Research Aircraft (HALO). The campaign took place in September-October 2014, with the objective of studying tropical deep convective clouds over the Amazon rainforest and their interactions with atmospheric trace gases, aerosol particles, and atmospheric radiation. Aerosol enhancements were observed consistently on all flights during which the UT was probed, using several aerosol metrics, including condensation nuclei (CN) and cloud condensation nuclei (CCN) number concentrations and chemical species mass concentrations. The UT particles differed sharply in their chemical composition and size distribution from those in the PBL, ruling out convective transport of combustion-derived particles from the boundary layer (BL) as a source. The air in the immediate outflow of deep convective clouds was depleted of aerosol particles, whereas strongly enhanced number concentrations of small particles ( 90 nm) particles in the UT, which consisted mostly of organic matter and nitrate and were very effective CCN. Our findings suggest a conceptual model, where production of new aerosol particles takes place in the continental UT from biogenic volatile organic material brought up by deep convection and converted to condensable

  19. Sulfur dioxide (SO2 from MIPAS in the upper troposphere and lower stratosphere 2002–2012

    Directory of Open Access Journals (Sweden)

    M. Höpfner

    2015-06-01

    Full Text Available Vertically resolved distributions of sulfur dioxide (SO2 with global coverage in the height region from the upper troposphere to ~20 km altitude have been derived from observations by the Michelson Interferometer for Passive Atmospheric Sounding (MIPAS on Envisat for the period July 2002 to April 2012. Retrieved volume mixing ratio profiles representing single measurements are characterized by typical errors in the range of 70–100 pptv and by a vertical resolution ranging from 3 to 5 km. Comparison with observations by the Atmospheric Chemistry Experiment Fourier transform spectrometer (ACE-FTS revealed a slightly varying bias with altitude of −20 to 50 pptv for the MIPAS data set in case of volcanically enhanced concentrations. For background concentrations the comparison showed a systematic difference between the two major MIPAS observation periods. After debiasing, the difference could be reduced to biases within −10 to 20 pptv in the altitude range of 10–20 km with respect to ACE-FTS. Further comparisons of the debiased MIPAS data set with in situ measurements from various aircraft campaigns showed no obvious inconsistencies within a range of around ±50 pptv. The SO2 emissions of more than 30 volcanic eruptions could be identified in the upper troposphere and lower stratosphere (UTLS. Emitted SO2 masses and lifetimes within different altitude ranges in the UTLS have been derived for a large part of these eruptions. Masses are in most cases within estimations derived from other instruments. From three of the major eruptions within the MIPAS measurement period – Kasatochi in August 2008, Sarychev in June 2009 and Nabro in June 2011 – derived lifetimes of SO2 for the altitude ranges 10–14, 14–18 and 18–22 km are 13.3 ± 2.1, 23.6 ± 1.2 and 32.3 ± 5.5 days respectively. By omitting periods with obvious volcanic influence we have derived background mixing ratio distributions of SO2. At 10 km altitude these indicate an annual

  20. A distribution law for relative humidity in the upper troposphere and lower stratosphere derived from three years of MOZAIC measurements

    Directory of Open Access Journals (Sweden)

    K. Gierens

    1999-09-01

    Full Text Available Data from three years of MOZAIC measurements made it possible to determine a distribution law for the relative humidity in the upper troposphere and lower stratosphere. Data amounting to 13.5% of the total were obtained in regions with ice supersaturation. Troposphere and stratosphere are distinguished by an ozone concentration of 130 ppbv as threshold. The probability of measuring a certain amount of ice supersaturation in the troposphere decreases exponentially with the degree of ice supersaturation. The probability of measuring a certain relative humidity in the stratosphere (both with respect to water and ice decreases exponentially with the relative humidity. A stochastic model that naturally leads to the exponential distribution is provided. Mean supersaturation in the troposphere is about 15%, whereas ice nucleation requires 30% supersaturation on the average. This explains the frequency of regions in which aircraft induce persistent contrails but which are otherwise free of clouds. Ice supersaturated regions are 3-4 K colder and contain more than 50% more vapour than other regions in the upper troposphere. The stratospheric air masses sampled are dry, as expected, having mean relative humidity over water of 12% and over ice of 23%, respectively. However, 2% of the stratospheric data indicate ice supersaturation. As the MOZAIC measurements have been obtained on commercial flights mainly between Europe and North America, the data do not provide a complete global picture, but the exponential character of the distribution laws found is probably valid globally. Since water vapour is the most important greenhouse gas and since it might enhance the anthropogenic greenhouse effects via positive feedback mechanisms, it is important to represent its distribution correctly in climate models. The discovery of the distribution law of the relative humidity makes possible simple tests to show whether the hydrological cycle in climate models is

  1. Concentrations of ethane (C2H6) in the lower stratosphere and upper troposphere and acetylene (C2H2) in the upper troposphere deduced from Atmospheric Trace Molecule Spectroscopy/Spacelab 3 spectra

    Science.gov (United States)

    Rinsland, C. P.; Russell, J. M., III; Zander, R.; Farmer, C. B.; Norton, R. H.

    1987-01-01

    This paper reports the results of the spectroscopic analysis of C2H6 and C2H2 absorption spectra obtained by the Atmospheric Trace Molecule Spectroscopy (ATMOS) instrument flown on the Shuttle as part of the Spacelab 3 mission. The spectra were recorded during sunset occultations occurring between 25 deg N and 31 deg N latitudes, yielding volume-mixing ratio profiles of C2H6 in the lower stratosphere and the upper troposphere, and an upper tropospheric profile of C2H2. These results compare well with previous in situ and remote sounding data obtained at similar latitudes and with model calculations. The results demonstrate the feasibility of the ATMOS instrument to sound the lower atmosphere from space.

  2. The representation of tropical upper tropospheric water in EC Earth V2

    Energy Technology Data Exchange (ETDEWEB)

    Johnston, M.S. [Chalmers University of Technology, Department of Earth and Space Sciences, Goeteburg (Sweden); Swedish Meteorological and Hydrological Institute (SMHI), Norrkoeping (Sweden); Eriksson, P.; Murtagh, D.P. [Chalmers University of Technology, Department of Earth and Space Sciences, Goeteburg (Sweden); Eliasson, S. [Luleaa University of Technology, Department of Computer Science, Electrical and Space Engineering, Kiruna (Sweden); Jones, C.G. [Swedish Meteorological and Hydrological Institute (SMHI), Norrkoeping (Sweden); Forbes, R.M. [ECMWF, Reading, Berkshire (United Kingdom)

    2012-12-15

    Tropical upper tropospheric humidity, clouds, and ice water content, as well as outgoing longwave radiation (OLR), are evaluated in the climate model EC Earth with the aid of satellite retrievals. The Atmospheric Infrared Sounder and Microwave Limb Sounder together provide good coverage of relative humidity. EC Earth's relative humidity is in fair agreement with these observations. CloudSat and CALIPSO data are combined to provide cloud fractions estimates throughout the altitude region considered (500-100 hPa). EC Earth is found to overestimate the degree of cloud cover above 200 hPa and underestimate it below. Precipitating and non-precipitating EC Earth ice definitions are combined to form a complete ice water content. EC Earth's ice water content is below the uncertainty range of CloudSat above 250 hPa, but can be twice as high as CloudSat's estimate in the melting layer. CERES data show that the model underestimates the impact of clouds on OLR, on average with about 9 W m{sup -2}. Regionally, EC Earth's outgoing longwave radiation can be {proportional_to}20 W m{sup -2} higher than the observation. A comparison to ERA-Interim provides further perspectives on the model's performance. Limitations of the satellite observations are emphasised and their uncertainties are, throughout, considered in the analysis. Evaluating multiple model variables in parallel is a more ambitious approach than is customary. (orig.)

  3. Retrieval of water vapor vertical distributions in the upper troposphere and the lower stratosphere from SCIAMACHY limb measurements

    OpenAIRE

    Rozanov, A.; Weigel, K.; Bovensmann, H.; Dhomse, S.; Eichmann, K.-U.; Kivi, R.; Rozanov, V.; Vömel, H.; Weber, M.; Burrows, J. P.

    2011-01-01

    This study describes the retrieval of water vapor vertical distributions in the upper troposphere and lower stratosphere (UTLS) altitude range from space-borne observations of the scattered solar light made in limb viewing geometry. First results using measurements from SCIAMACHY (Scanning Imaging Absorption spectroMeter for Atmospheric CHartographY) aboard ENVISAT (Environmental Satellite) are presented here. In previous publications, the retrieval of water vapor vertical ...

  4. Summertime mid-to-upper tropospheric nitrous oxide over the Mediterranean as a footprint of Indian emissions

    Science.gov (United States)

    Kangah, Yannick; Ricaud, Philippe; Attié, Jean-Luc; Saitoh, Naoko; Hauglustaine, Didier; El Amraoui, Laaziz; Zbinden, Regina; Delon, Claire

    2016-04-01

    We used global scale thermal infrared measurements of mid-to-upper tropospheric nitrous oxide (N2O) from the Greenhouse gases Observing SATellite (GOSAT) and outputs from the 3D Chemical Transport Model LMDz-OR-INCA to assess the impact of the Indian subcontinent N2O emissions on the N2O field over the eastern Mediterranean Basin (MB) during summer. The use of nitrogen fertilizer coupled with high soil humidity during summer monsoon period produce high emissions of N2O in many south Asian countries and especially the Indian subcontinent. N2O is transported to the upper troposphere by updrafts associated to the monsoon and redistributed westward to the eastern Mediterranean via the Asian Monsoon Anticyclone. This summertime (June-July-August) enrichment in N2O in the eastern Mediterranean produces a maximum in the east-west difference of MB mid-to-upper tropospheric N2O anomaly representative for the period 2010-2013 with a maximum in July and a peak-to-peak amplitude of ~1.0 ± 0.3 ppbv observed by GOSAT consistently with LMDz-OR-INCA but less intense (~0.5 ppbv). This summertime enrichment of N2O over the eastern Mediterranean is consistent with the increase of the surface emissions and the convective precipitations over the Indian subcontinent during the summer monsoon period. N2O over the eastern Mediterranean can therefore be considered as a footprint of Indian summertime emissions.

  5. Towards a Model Climatology of Relative Humidity in the Upper Troposphere for Estimation of Contrail and Contrail-Induced Cirrus

    Science.gov (United States)

    Selkirk, Henry B.; Manyin, M.; Ott, L.; Oman, L.; Benson, C.; Pawson, S.; Douglass, A. R.; Stolarski, R. S.

    2011-01-01

    The formation of contrails and contrail cirrus is very sensitive to the relative humidity of the upper troposphere. To reduce uncertainty in an estimate of the radiative impact of aviation-induced cirrus, a model must therefore be able to reproduce the observed background moisture fields with reasonable and quantifiable fidelity. Here we present an upper tropospheric moisture climatology from a 26-year ensemble of simulations using the GEOS CCM. We compare this free-running model's moisture fields to those obtained from the MLS and AIRS satellite instruments, our most comprehensive observational databases for upper tropospheric water vapor. Published comparisons have shown a substantial wet bias in GEOS-5 assimilated fields with respect to MLS water vapor and ice water content. This tendency is clear as well in the GEOS CCM simulations. The GEOS-5 moist physics in the GEOS CCM uses a saturation adjustment that prevents supersaturation, which is unrealistic when compared to in situ moisture observations from MOZAIC aircraft and balloon sondes as we will show. Further, the large-scale satellite datasets also consistently underestimate super-saturation when compared to the in-situ observations. We place these results in the context of estimates of contrail and contrail cirrus frequency.

  6. Hydrogen Cyanide in the Upper Troposphere: GEM-AQ Simulation and Comparison with ACE-FTS Observations

    Science.gov (United States)

    Lupu, A.; Kaminski, J. W.; Neary, L.; McConnell, J. C.; Toyota, K.; Rinsland, C. P.; Bernath, P. F.; Walker, K. A.; Boone, C. D.; Nagahama, Y.; hide

    2009-01-01

    We investigate the spatial and temporal distribution of hydrogen cyanide (HCN) in the upper troposphere through numerical simulations and comparison with observations from a space-based instrument. To perform the simulations, we used the Global Environmental Multiscale Air Quality model (GEM-AQ), which is based on the threedimensional Gobal multiscale model developed by the Meteorological Service of Canada for operational weather forecasting. The model was run for the period 2004-2006 on a 1.5deg x 1.5deg global grid with 28 hybrid vertical levels from the surface up to 10 hPa. Objective analysis data from the Canadian Meteorological Centre were used to update the meteorological fields every 24 h. Fire emission fluxes of gas species were generated by using year-specific inventories of carbon emissions with 8-day temporal resolution from the Global Fire Emission Database (GFED) version 2. The model output is compared with HCN profiles measured by the Atmospheric Chemistry Experiment Fourier Transform Spectrometer (ACE-FTS) instrument onboard the Canadian SCISAT-1 satellite. High values of up to a few ppbv are observed in the tropics in the Southern Hemisphere; the enhancement in HCN volume mixing ratios in the upper troposphere is most prominent in October. Low upper-tropospheric mixing ratios of less than 100 pptv are mostly recorded at middle and high latitudes in the Southern Hemisphere in May-July. Mixing ratios in Northern Hemisphere peak in the boreal summer. The amplitude of the seasonal variation is less pronounced than in the Southern Hemisphere. The comparison with the satellite data shows that in the upper troposphere GEM-AQ perform7s well globally for all seasons, except at northern hi gh and middle latitudes in surnmer, where the model has a large negative bias, and in the tropics in winter and spring, where it exhibits large positive bias. This may reflect inaccurate emissions or possible inaccuracies in the emission profile. The model is able to

  7. The Effect of Cirrus Clouds on Water Vapor Transport in the Upper Troposphere and Lower Stratosphere

    Science.gov (United States)

    Lei, L.; McCormick, M. P.; Anderson, J.

    2017-12-01

    Water vapor plays an important role in the Earth's radiation budget and stratospheric chemistry. It is widely accepted that a large percentage of water vapor entering the stratosphere travels through the tropical tropopause and is dehydrated by the cold tropopause temperature. The vertical transport of water vapor is also affected by the radiative effects of cirrus clouds in the tropical tropopause layer. This latter effect of cirrus clouds was investigated in this research. The work focuses on the tropical and mid-latitude region (50N-50S). Water vapor data from the Microwave Limb Sounder (MLS) and cirrus cloud data from the Cloud-Aerosol Lidar and Infrared pathfinder Satellite Observation (CALIPSO) instruments were used to investigate the relationship between the water vapor and the occurrence of cirrus cloud. A 10-degree in longitude by 10-degree in latitude resolution was chosen to bin the MLS and CALIPSO data. The result shows that the maximum water vapor in the upper troposphere (below 146 hPa) is matched very well with the highest frequency of cirrus cloud occurrences. Maximum water vapor in the lower stratosphere (100 hPa) is partly matched with the maximum cirrus cloud occurrence in the summer time. The National Oceanic and Atmospheric Administration Interpolated Outgoing Longwave Radiation data and NCEP-DOE Reanalysis 2 wind data were used also to investigate the relationship between the water vapor entering the stratosphere, deep convection, and wind. Results show that maximum water vapor at 100 hPa coincides with the northern hemisphere summer-time anticyclone. The effects from both single-layer cirrus clouds and cirrus clouds above the anvil top on the water vapor entering the stratosphere were also studied and will be presented.

  8. Two-dimensional performance of MIPAS observation modes in the upper-troposphere/lower-stratosphere

    Directory of Open Access Journals (Sweden)

    M. Carlotti

    2011-02-01

    Full Text Available In this paper we analyze the performance of the three MIPAS (Michelson Interferometer for Passive Atmospheric Sounding observation modes that sound the Upper-Troposphere/Lower-Stratosphere (UT/LS region. The two-dimensional (2-D tomographic retrieval approach is assumed to derive the atmospheric field of geophysical parameters. For each observation mode we have calculated the 2-D distribution of the information load quantifier relative to the main MIPAS targets. The performance of the observation modes has been evaluated in terms of strength and spatial coverage of the information-load distribution along the full orbit. The indications of the information-load analysis has been validated with simulated retrievals based on the observational parameters of real orbits. In the simulation studies we have assessed the precision and the spatial (both horizontal and vertical resolution of the retrieval products. The performance of the three observation modes has been compared for the MIPAS main products in both the UT/LS and the extended altitude range. This study shows that the two observation modes that were specifically designed for the UT/LS region are actually competitive with the third one, designed for the whole stratosphere, up to altitudes that far exceed the UT/LS. In the UT/LS the performance of the two specific observation modes is comparable even if the best performance in terms of horizontal resolution is provided by the observation mode that was excluded by the European Space Agency (ESA from the current MIPAS duty cycle. This paper reports the first application of the information-load analysis and highlights the worthiness of this approach to make qualitative considerations about retrieval potential and selection of retrieval grid.

  9. NOAA Climate Data Record for Mean Layer Temperature (Upper Troposphere & Lower Stratosphere) from UCAR, Version 2

    Data.gov (United States)

    National Oceanic and Atmospheric Administration, Department of Commerce — The Temperatures of Troposphere / Stratosphere (TTS) (AMSU channel 7 and MSU channel 3) CDR is generated by using National Oceanic and Atmospheric Administration...

  10. Evaluation of Satellite-Based Upper Troposphere Cloud Top Height Retrievals in Multilayer Cloud Conditions During TC4

    Science.gov (United States)

    Chang, Fu-Lung; Minnis, Patrick; Ayers, J. Kirk; McGill, Matthew J.; Palikonda, Rabindra; Spangenberg, Douglas A.; Smith, William L., Jr.; Yost, Christopher R.

    2010-01-01

    Upper troposphere cloud top heights (CTHs), restricted to cloud top pressures (CTPs) less than 500 hPa, inferred using four satellite retrieval methods applied to Twelfth Geostationary Operational Environmental Satellite (GOES-12) data are evaluated using measurements during the July August 2007 Tropical Composition, Cloud and Climate Coupling Experiment (TC4). The four methods are the single-layer CO2-absorption technique (SCO2AT), a modified CO2-absorption technique (MCO2AT) developed for improving both single-layered and multilayered cloud retrievals, a standard version of the Visible Infrared Solar-infrared Split-window Technique (old VISST), and a new version of VISST (new VISST) recently developed to improve cloud property retrievals. They are evaluated by comparing with ER-2 aircraft-based Cloud Physics Lidar (CPL) data taken during 9 days having extensive upper troposphere cirrus, anvil, and convective clouds. Compared to the 89% coverage by upper tropospheric clouds detected by the CPL, the SCO2AT, MCO2AT, old VISST, and new VISST retrieved CTPs less than 500 hPa in 76, 76, 69, and 74% of the matched pixels, respectively. Most of the differences are due to subvisible and optically thin cirrus clouds occurring near the tropopause that were detected only by the CPL. The mean upper tropospheric CTHs for the 9 days are 14.2 (+/- 2.1) km from the CPL and 10.7 (+/- 2.1), 12.1 (+/- 1.6), 9.7 (+/- 2.9), and 11.4 (+/- 2.8) km from the SCO2AT, MCO2AT, old VISST, and new VISST, respectively. Compared to the CPL, the MCO2AT CTHs had the smallest mean biases for semitransparent high clouds in both single-layered and multilayered situations whereas the new VISST CTHs had the smallest mean biases when upper clouds were opaque and optically thick. The biases for all techniques increased with increasing numbers of cloud layers. The transparency of the upper layer clouds tends to increase with the numbers of cloud layers.

  11. Carbon monoxide distributions from the upper troposphere to the mesosphere inferred from 4.7 μm non-local thermal equilibrium emissions measured by MIPAS on Envisat

    Directory of Open Access Journals (Sweden)

    B. Funke

    2009-04-01

    Full Text Available We present global distributions of carbon monoxide (CO from the upper troposphere to the mesosphere observed by the Michelson Interferometer for Passive Atmospheric Sounding (MIPAS on Envisat. Vertically resolved volume mixing ratio profiles have been retrieved from 4.7 μm limb emission spectra under consideration of non-local thermodynamic equilibrium. The precision of individual CO profiles is typically 5–30 ppbv (15–40% for altitudes greater than 40 km and lower than 15 km and 30–90% within 15–40 km. Estimated systematic errors are in the order of 8–15%. Below 60 km, the vertical resolution is 4–7 km. The data set which covers 54 days from September 2003 to March 2004 has been derived with an improved retrieval version including (i the retrieval of log(vmr, (ii the consideration of illumination-dependent vibrational population gradients along the instrument's line of sight, and (iii joint-fitted vmr horizontal gradients in latitudinal and longitudinal directions. A detailed analysis of spatially resolved CO distributions during the 2003/2004 Northern Hemisphere major warming event demonstrate the potential of MIPAS CO observations to obtain new information on transport processes during dynamical active episodes, particularly on those acting in the vertical. From the temporal evolution of zonally averaged CO abundances, we derived extraordinary polar winter descent velocities of 1200 m per day inside the recovered polar vortex in January 2004. Middle stratospheric CO abundances show a well established correlation with the chemical source CH4, particularly in the tropics. In the upper troposphere, a moderate CO decrease from September 2003 to March 2004 was observed. Upper tropospheric CO observations provide a detailed picture of long-range transport of polluted air masses and uplift events. MIPAS observations taken on 9–11 September 2003 confirm the trapping of convective outflow of polluted CO-rich air from

  12. Acetylene C2H 2 retrievals from MIPAS data and regions of enhanced upper tropospheric concentrations in August 2003

    Directory of Open Access Journals (Sweden)

    V. P. Kanawade

    2011-10-01

    Full Text Available Acetylene (C2H2 volume mixing ratios (VMRs have been successfully retrieved from the Michelson Interferometer for Passive Atmospheric Sounding (MIPAS Level 1B radiances during August 2003, providing the first global map of such data and ratios to CO in the literature. The data presented here contain most information between 300 hPa and 100 hPa with systematic errors less than 10% at the upper levels. Random errors per point are less than 15% at lower levels and are closer to 30% at 100 hPa. Global distributions of the C2H2 and C2H2/CO ratio confirm significant features associated with both the Asian monsoon anticyclone and biomass burning for this important hydrocarbon in a characteristic summer month (August 2003, showing tight correlations regionally, particularly at lower to medium values, but globally emphasising the differences between sources and lifetimes of CO and C2H2. The correlations are seen to be particularly disturbed in the regions of highest C2H2 concentrations, indicating variability in the surface emissions or fast processing. A strong isolation of C2H2 within the Asian monsoon anticyclone is observed, evidencing convective transport into the upper troposphere, horizontal advection within the anticyclone at 200 hPa, distinct gradients at the westward edge of the vortex and formation of a secondary dynamical feature from the eastward extension of the anticyclone outflow over the Asian Pacific. Ratios of C2H2/CO are consistent with the evidence from the cross-sections that the C2H2 is uplifted rapidly in convection. Observations are presented of enhanced C2H2 associated with the injection from biomass burning into the upper troposphere and the outflow from Africa at 200 hPa into both the Atlantic and Indian Oceans. In the biomass burning regions, C2H2 and CO are well correlated, but the uplift is less marked and peaks at lower altitudes compared to the strong effects observed in the Asian monsoon anticyclone. Ratios of C2H2/CO

  13. Mid-upper tropospheric methane retrieval from IASI and its validation

    Directory of Open Access Journals (Sweden)

    X. Xiong

    2013-09-01

    Full Text Available Mid-upper tropospheric methane (CH4, as an operational product at NOAA's (National Oceanic and Atmospheric Administration Comprehensive Large Array-data Stewardship System (CLASS, has been retrieved from the Infrared Atmospheric Sounding Interferometer (IASI since 2008. This paper provides a description of the retrieval method and the validation using 596 CH4 vertical profiles from aircraft measurements by the HIAPER Pole-to-Pole Observations (HIPPO program over the Pacific Ocean. The number of degrees of freedom for the CH4 retrieval is mostly less than 1.5, and it decreases under cloudy conditions. The retrievals show greatest sensitivity between 100–600 hPa in the tropics and 200–750 hPa in the mid- to high latitude. Validation is accomplished using aircraft measurements (convolved by applying the monthly mean averaging kernels collocated with all the retrieved profiles within 200 km and on the same day, and the results show that, on average, a larger error of CH4 occurs at 300–500 hPa. The bias in the trapezoid of 374–477 hPa is −1.74% with a residual standard deviation of 1.20%, and at layer 596–753 hPa the bias is −0.69% with a residual standard deviation of 1.07%. The retrieval error is relatively larger in the high northern latitude regions and/or under cloudy conditions. The main reasons for this negative bias include the uncertainty in the spectroscopy near the methane Q branch and/or the empirical bias correction, plus residual cloud contamination in the cloud-cleared radiances. It is expected for NOAA to generate the CH4 product for 20 + years using a similar algorithm from three similar thermal infrared sensors: Atmospheric Infrared Sounder (AIRS, IASI and the Cross-track Infrared Sounder (CrIS. Such a unique product will provide a supplementary to the current ground-based observation network, particularly in the Arctic, for monitoring the CH4 cycle, its transport and trend associated with climate change.

  14. Momentum flux associated with gravity waves in the low-latitude troposphere

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    S. R. Prabhakaran Nayar

    Full Text Available The vertical fluxes of horizontal momentum at tropospheric heights are calculated for four days, 25–28 August 1999. The mean zonal wind during these days show the presence of strong westward wind at the upper troposphere. Both the symmetric beam radar method and the power spectral method of evaluation of vertical flux of zonal and meridional momentum shows nearly the same result for quiet conditions. The temporal evolution of the momentum flux is estimated for a day with strong zonal shear and convection. These results indicate that on 28 August 1999, the strong downward vertical wind in the lower altitude range is associated with upward vertical flux of zonal momentum, and strong upward vertical wind is associated with downward vertical flux. Similarly, the strong shear in zonal wind is associated with the increase in negative values in vertical flux in the upper troposphere. Analysis of the role of wave periods in the transport of momentum flux indicates that the vertical momentum flux magnitude is not evenly distributed in all wave periods, but instead it peaks at certain wave periods in the range 10 to 100 min.

    Key words. Meteorology and atmospheric dynamics (convective process; tropical meteorology; precipitation

  15. The Relative Importance of Random Error and Observation Frequency in Detecting Trends in Upper Tropospheric Water Vapor

    Science.gov (United States)

    Whiteman, David N.; Vermeesch, Kevin C.; Oman, Luke D.; Weatherhead, Elizabeth C.

    2011-01-01

    Recent published work assessed the amount of time to detect trends in atmospheric water vapor over the coming century. We address the same question and conclude that under the most optimistic scenarios and assuming perfect data (i.e., observations with no measurement uncertainty) the time to detect trends will be at least 12 years at approximately 200 hPa in the upper troposphere. Our times to detect trends are therefore shorter than those recently reported and this difference is affected by data sources used, method of processing the data, geographic location and pressure level in the atmosphere where the analyses were performed. We then consider the question of how instrumental uncertainty plays into the assessment of time to detect trends. We conclude that due to the high natural variability in atmospheric water vapor, the amount of time to detect trends in the upper troposphere is relatively insensitive to instrumental random uncertainty and that it is much more important to increase the frequency of measurement than to decrease the random error in the measurement. This is put in the context of international networks such as the Global Climate Observing System (GCOS) Reference Upper-Air Network (GRUAN) and the Network for the Detection of Atmospheric Composition Change (NDACC) that are tasked with developing time series of climate quality water vapor data.

  16. Inertia gravity waves in the upper troposphere during the MaCWAVE winter campaign. Part I. Observations with collocated radars

    Energy Technology Data Exchange (ETDEWEB)

    Hoffmann, P.; Serafimovich, A.; Peters, D.; Latteck, R. [Leibniz-Inst. fuer Atmosphaerenphysik, Kuehlungsborn (Germany); Dalin, P. [Swedish Inst. of Space Physics, Kiruna (Sweden); Goldberg, R. [NASA/Goddard Space Flight Center, Greenbelt, MD (United States)

    2006-07-01

    During the MaCWAVE campaign, combined rocket, radiosonde and ground-based measurements have been performed at the Norwegian Andoeya rocket range (ARR) near Andenes and the Swedish rocket range (ESRANGE) near Kiruna in January 2003 to study gravity waves in the vicinity of the Scandinavian mountain ridge. The investigations presented here are mainly based on the evaluation of continuous radar measurements with the ALWIN VHP radar in the upper troposphere/ lower stratosphere at Andenes (69.3 N, 16.0 E) and the ESRAD VHP radar near Kiruna (67.9 N, 21.9 E). Both radars are separated by about 260 km. Based on wavelet transformations of both data sets, the strongest activity of inertia gravity waves in the upper troposphere has been detected during the first period from 24-26 January 2003 with dominant vertical wavelengths of about 4-5 km as well as with dominant observed periods of about 13-14 h for the altitude range between 5 and 8 km under the additional influence of mountain waves. The results show the appearance of dominating inertia gravity waves with characteristic horizontal wavelengths of {proportional_to}200 km moving in the opposite direction than the mean background wind. The results show the appearance of dominating inertia gravity waves with intrinsic periods in the order of {proportional_to}5 h and with horizontal wavelengths of 200 km, moving in the opposite direction than the mean background wind. From the derived downward energy propagation it is supposed, that these waves are likely generated by a jet streak in the upper troposphere. The parameters of the jet-induced gravity waves have been estimated at both sites separately. The identified gravity waves are coherent at both locations and show higher amplitudes on the east-side of the Scandinavian mountain ridge, as expected by the influence of mountains. (orig.)

  17. Dynamics in the Modern Upper Atmosphere of Venus: Zonal Wind Transition to Subsolar-to-Antisolar Flow

    Science.gov (United States)

    Livengood, T. A.; Kostiuk, T.; Hewagama, T.; Fast, K. E.

    2017-12-01

    We observed Venus on 19-23 Aug 2010 (UT) to investigate equatorial wind velocities from above the cloud tops through the lower thermosphere. Measurements were made from the NASA Infrared Telescope Facility using the NASA Goddard Space Flight Center Heterodyne Instrument for Planetary Winds and Composition. High-resolution spectra were acquired on a CO2 pressure-broadened absorption feature that probes the lower mesosphere ( 70 km altitude) with a non-LTE core emission of the same transition that probes the lower thermosphere ( 110 km). The resolving power of λ/Δλ≈3×107 determines line-of-sight velocity from Doppler shifts to high precision. The altitude differential between the features enables investigating the transition from zonal wind flow near the cloud tops to subsolar-to-antisolar flow in the thermosphere. The fully-resolved carbon dioxide transition was measured near 952.8808 cm-1 (10.494 µm) rest frequency at the equator with 1 arcsec field-of-view on Venus (24 arcsec diameter) distributed about the central meridian and across the terminator at ±15° intervals in longitude. The non-LTE emission is solar-pumped and appears only on the daylight side, probing subsolar-to-antisolar wind velocity vector flowing radially from the subsolar point through the terminator, which was near the central meridian in these observations and had zero line-of-sight wind projection at the terminator. The velocity of the zonal flow is approximately uniform, with maximum line-of-sight projection at the limb, and can be measured by the frequency of the absorption line on both the daylight and dark side. Variations in Doppler shift between the observable features and the differing angular dependence of the contributing wind phenomena thus provide independent mechanisms to distinguish the dynamical processes at the altitude of each observed spectral feature. Winds up to >100 m/s were determined in previous investigations with uncertainties of order 10 m/s or less.

  18. A large impact of tropical biomass burning on CO and CO{sub 2} in the upper troposphere

    Energy Technology Data Exchange (ETDEWEB)

    Hidekazu Matsueda; Shoichi Taguchi; Hisayuki Y; Inoue & Masao Ishii [Meteorological Research Institute, Tsukuba-shi (Japan). Geochemical Research Department

    2002-07-01

    A large interannual variation of biomass burning emissions from Southeast Asia is associated with the ENSO events. During 1997/98 and 1994 El Nino years, uncontrolled wildfires of tropical rainforests and peat lands in Indonesia were enlarged due to a long drought. Enhanced CO injection into the upper troposphere from the intense Indonesian fires was clearly observed in the 8-year measurements from a regular flask sampling over the western Pacific using a JAL airliner between Australia and Japan. This airliner observation also revealed that upper tropospheric CO{sub 2} cycle largely changed during the 1997 El Nio year due partly to the biomass burning emissions. Widespread pollution from the biomass burnings in Southeast Asia was simulated using a CO tracer driven by a 3D global chemical transport model. This simulation indicates that tropical deep convections connected to rapid advection by the subtropical jet play a significant role in dispersing biomass-burning emissions from Southeast Asia on a global scale.

  19. An upper tropospheric ‘ozone river’ from Africa to India during the 2008 Asian post-monsoon season

    Directory of Open Access Journals (Sweden)

    Flore Tocquer

    2015-03-01

    Full Text Available We have used ozone data from the Infrared Atmospheric Sounding Interferometer to follow an event of ozone-enriched air-masses in the upper troposphere from eastern Africa to northern India. The ozone transport (hereafter called ‘ozone river’ or O3R occurred during the Asian post-monsoon season in 2008 and was associated with Rossby wave propagation. The persistence of the O3R in a narrow channel was confirmed by MOZAIC airborne data over the northwestern Indian coast. The regions of origin of the O3R were identified by a transport analysis based on the Lagrangian model FLEXPART. The Lagrangian simulations combined with potential vorticity fields indicate that stratospheric intrusions are not likely to be the most important contributor to the observed O3 enhancements. A high-resolution Eulerian model, Meso-NH, with tagged tracers was used to discriminate between African biomass burning, lightnings and Indian anthropogenic pollution as potential sources of precursors for the O3R. Lightning NOx emissions, associated with convective clouds over Africa, were found to be the principal contributor to the ozone enhancement over the Indian Ocean taking advantage of a northeastward jet. This case study illustrates African lightning emissions as an important source for enhanced O3 in the upper troposphere over the Indian Ocean region during the post-monsoon season.

  20. Regular in situ measurements of HDO/H216O in the northern and southern hemispherical upper troposphere reveal tropospheric transport processes.

    Science.gov (United States)

    Christner, Emanuel; Dyroff, Christoph; Sanati, Shahrokh; Brenninkmeijer, Carl; Zahn, Andreas

    2013-04-01

    influence of convection on the isotopic composition of water in the upper troposphere. This finding is consistent with the well-known regions of deep convection over Africa, Malaysia and South America.

  1. Satellite observations and modeling of transport in the upper troposphere through the lower mesosphere during the 2006 major stratospheric sudden warming

    Directory of Open Access Journals (Sweden)

    W. H. Daffer

    2009-07-01

    Full Text Available An unusually strong and prolonged stratospheric sudden warming (SSW in January 2006 was the first major SSW for which globally distributed long-lived trace gas data are available covering the upper troposphere through the lower mesosphere. We use Aura Microwave Limb Sounder (MLS, Atmospheric Chemistry Experiment-Fourier Transform Spectrometer (ACE-FTS data, the SLIMCAT Chemistry Transport Model (CTM, and assimilated meteorological analyses to provide a comprehensive picture of transport during this event. The upper tropospheric ridge that triggered the SSW was associated with an elevated tropopause and layering in trace gas profiles in conjunction with stratospheric and tropospheric intrusions. Anomalous poleward transport (with corresponding quasi-isentropic troposphere-to-stratosphere exchange at the lowest levels studied in the region over the ridge extended well into the lower stratosphere. In the middle and upper stratosphere, the breakdown of the polar vortex transport barrier was seen in a signature of rapid, widespread mixing in trace gases, including CO, H2O, CH4 and N2O. The vortex broke down slightly later and more slowly in the lower than in the middle stratosphere. In the middle and lower stratosphere, small remnants with trace gas values characteristic of the pre-SSW vortex lingered through the weak and slow recovery of the vortex. The upper stratospheric vortex quickly reformed, and, as enhanced diabatic descent set in, CO descended into this strong vortex, echoing the fall vortex development. Trace gas evolution in the SLIMCAT CTM agrees well with that in the satellite trace gas data from the upper troposphere through the middle stratosphere. In the upper stratosphere and lower mesosphere, the SLIMCAT simulation does not capture the strong descent of mesospheric CO and H2O values into the reformed vortex; this poor CTM performance in the upper stratosphere and lower mesosphere results

  2. A modelling study of the impact of cirrus clouds on the moisture budget of the upper troposphere

    Directory of Open Access Journals (Sweden)

    S. Fueglistaler

    2006-01-01

    Full Text Available We present a modelling study of the effect of cirrus clouds on the moisture budget of the layer wherein the cloud formed. Our framework simplifies many aspects of cloud microphysics and collapses the problem of sedimentation onto a 0-dimensional box model, but retains essential feedbacks between saturation mixing ratio, particle growth, and water removal through particle sedimentation. The water budget is described by two coupled first-order differential equations for dimensionless particle number density and saturation point temperature, where the parameters defining the system (layer depth, reference temperature, amplitude and time scale of temperature perturbation and inital particle number density, which may or may not be a function of reference temperature and cooling rate are encapsulated in a single coefficient. This allows us to scale the results to a broad range of atmospheric conditions, and to test sensitivities. Results of the moisture budget calculations are presented for a range of atmospheric conditions (T: 238–205 K; p: 325–180 hPa and a range of time scales τT of the temperature perturbation that induces the cloud formation. The cirrus clouds are found to efficiently remove water for τT longer than a few hours, with longer perturbations (τT≳10 h required at lower temperatures (T≲210 K. Conversely, we find that temperature perturbations of duration order 1 h and less (a typical timescale for e.g., gravity waves do not efficiently dehydrate over most of the upper troposphere. A consequence is that (for particle densities typical of current cirrus clouds the assumption of complete dehydration to the saturation mixing ratio may yield valid predictions for upper tropospheric moisture distributions if it is based on the large scale temperature field, but this assumption is not necessarily valid if it is based on smaller scale temperature fields.

  3. Northern Winter Climate Change: Assessment of Uncertainty in CMIP5 Projections Related to Stratosphere-Troposphere Coupling

    Science.gov (United States)

    Manzini, E.; Karpechko, A.Yu.; Anstey, J.; Shindell, Drew Todd; Baldwin, M.P.; Black, R.X.; Cagnazzo, C.; Calvo, N.; Charlton-Perez, A.; Christiansen, B.; hide

    2014-01-01

    Future changes in the stratospheric circulation could have an important impact on northern winter tropospheric climate change, given that sea level pressure (SLP) responds not only to tropospheric circulation variations but also to vertically coherent variations in troposphere-stratosphere circulation. Here we assess northern winter stratospheric change and its potential to influence surface climate change in the Coupled Model Intercomparison Project-Phase 5 (CMIP5) multimodel ensemble. In the stratosphere at high latitudes, an easterly change in zonally averaged zonal wind is found for the majority of the CMIP5 models, under the Representative Concentration Pathway 8.5 scenario. Comparable results are also found in the 1% CO2 increase per year projections, indicating that the stratospheric easterly change is common feature in future climate projections. This stratospheric wind change, however, shows a significant spread among the models. By using linear regression, we quantify the impact of tropical upper troposphere warming, polar amplification, and the stratospheric wind change on SLP. We find that the intermodel spread in stratospheric wind change contributes substantially to the intermodel spread in Arctic SLP change. The role of the stratosphere in determining part of the spread in SLP change is supported by the fact that the SLP change lags the stratospheric zonally averaged wind change. Taken together, these findings provide further support for the importance of simulating the coupling between the stratosphere and the troposphere, to narrow the uncertainty in the future projection of tropospheric circulation changes.

  4. Large-scale upper tropospheric pollution observed by MIPAS HCN and C2H6 global distributions

    Science.gov (United States)

    Glatthor, N.; von Clarmann, T.; Stiller, G. P.; Funke, B.; Koukouli, M. E.; Fischer, H.; Grabowski, U.; Höpfner, M.; Kellmann, S.; Linden, A.

    2009-12-01

    We present global upper tropospheric HCN and C2H6 amounts derived from MIPAS/ENVISAT limb emission spectra. HCN and C2H6 are retrieved in the spectral regions 715.5-782.7 cm-1 and 811.5-835.7 cm-1, respectively. The datasets consist of 54 days between September 2003 and March 2004. This period covers the peak and decline of the southern hemispheric biomass burning period and some months thereafter. HCN is a nearly unambiguous tracer of biomass burning with an assumed tropospheric lifetime of several months. Indeed, the most significant feature in the MIPAS HCN dataset is an upper tropospheric plume of enhanced values caused by southern hemispheric biomass burning, which in September and October 2003 extended from tropical South America over Africa, Australia to the Southern Pacific. The spatial extent of this plume agrees well with the MOPITT CO distribution of September 2003. Further there is good agreement with the shapes and mixing ratios of the southern hemispheric HCN and C2H6 fields measured by the ACE experiment between September and November 2005. The MIPAS HCN plume extended from the lowermost observation height of 8 km up to about 16 km altitude, with maximum values of 500-600 pptv in October 2003. It was still clearly visible in December 2003, but had strongly decreased by March 2004, confirming the assumed tropospheric lifetime. The main sources of C2H6 are production and transmission of fossil fuels, followed by biofuel use and biomass burning. The C2H6 distribution also clearly reflected the southern hemispheric biomass burning plume and its seasonal variation, with maximum amounts of 600-700 pptv. Generally there was good spatial overlap between the southern hemispheric distributions of both pollution tracers, except for the region between Peru and the mid-Pacific. Here C2H6was considerably enhanced, whereas the HCN amounts were low. Backward trajectory calculations suggested that industrial pollution was responsible for the elevated C2H6

  5. Large-scale upper tropospheric pollution observed by MIPAS HCN and C2H6 global distributions

    Directory of Open Access Journals (Sweden)

    A. Linden

    2009-12-01

    Full Text Available We present global upper tropospheric HCN and C2H6 amounts derived from MIPAS/ENVISAT limb emission spectra. HCN and C2H6 are retrieved in the spectral regions 715.5–782.7 cm−1 and 811.5–835.7 cm−1, respectively. The datasets consist of 54 days between September 2003 and March 2004. This period covers the peak and decline of the southern hemispheric biomass burning period and some months thereafter. HCN is a nearly unambiguous tracer of biomass burning with an assumed tropospheric lifetime of several months. Indeed, the most significant feature in the MIPAS HCN dataset is an upper tropospheric plume of enhanced values caused by southern hemispheric biomass burning, which in September and October 2003 extended from tropical South America over Africa, Australia to the Southern Pacific. The spatial extent of this plume agrees well with the MOPITT CO distribution of September 2003. Further there is good agreement with the shapes and mixing ratios of the southern hemispheric HCN and C2H6 fields measured by the ACE experiment between September and November 2005. The MIPAS HCN plume extended from the lowermost observation height of 8 km up to about 16 km altitude, with maximum values of 500–600 pptv in October 2003. It was still clearly visible in December 2003, but had strongly decreased by March 2004, confirming the assumed tropospheric lifetime. The main sources of C2H6 are production and transmission of fossil fuels, followed by biofuel use and biomass burning. The C2H6 distribution also clearly reflected the southern hemispheric biomass burning plume and its seasonal variation, with maximum amounts of 600–700 pptv. Generally there was good spatial overlap between the southern hemispheric distributions of both pollution tracers, except for the region between Peru and the mid-Pacific. Here C2H6was considerably enhanced, whereas the HCN amounts were low. Backward trajectory calculations suggested that industrial pollution was responsible

  6. Assessment of upper tropospheric and stratospheric water vapor and ozone in reanalyses as part of S-RIP

    Science.gov (United States)

    Davis, Sean M.; Hegglin, Michaela I.; Fujiwara, Masatomo; Dragani, Rossana; Harada, Yayoi; Kobayashi, Chiaki; Long, Craig; Manney, Gloria L.; Nash, Eric R.; Potter, Gerald L.; Tegtmeier, Susann; Wang, Tao; Wargan, Krzysztof; Wright, Jonathon S.

    2017-10-01

    Reanalysis data sets are widely used to understand atmospheric processes and past variability, and are often used to stand in as "observations" for comparisons with climate model output. Because of the central role of water vapor (WV) and ozone (O3) in climate change, it is important to understand how accurately and consistently these species are represented in existing global reanalyses. In this paper, we present the results of WV and O3 intercomparisons that have been performed as part of the SPARC (Stratosphere-troposphere Processes and their Role in Climate) Reanalysis Intercomparison Project (S-RIP). The comparisons cover a range of timescales and evaluate both inter-reanalysis and observation-reanalysis differences. We also provide a systematic documentation of the treatment of WV and O3 in current reanalyses to aid future research and guide the interpretation of differences amongst reanalysis fields.The assimilation of total column ozone (TCO) observations in newer reanalyses results in realistic representations of TCO in reanalyses except when data coverage is lacking, such as during polar night. The vertical distribution of ozone is also relatively well represented in the stratosphere in reanalyses, particularly given the relatively weak constraints on ozone vertical structure provided by most assimilated observations and the simplistic representations of ozone photochemical processes in most of the reanalysis forecast models. However, significant biases in the vertical distribution of ozone are found in the upper troposphere and lower stratosphere in all reanalyses.In contrast to O3, reanalysis estimates of stratospheric WV are not directly constrained by assimilated data. Observations of atmospheric humidity are typically used only in the troposphere, below a specified vertical level at or near the tropopause. The fidelity of reanalysis stratospheric WV products is therefore mainly dependent on the reanalyses' representation of the physical drivers that

  7. Evaluating Lightning-generated NOx (LNOx) Parameterization based on Cloud Top Height at Resolutions with Partially-resolved Convection for Upper Tropospheric Chemistry Studies

    Science.gov (United States)

    Wong, J.; Barth, M. C.; Noone, D. C.

    2012-12-01

    Lightning-generated nitrogen oxides (LNOx) is an important precursor to tropospheric ozone production. With a meteorological time-scale variability similar to that of the ozone chemical lifetime, it can nonlinearly perturb tropospheric ozone concentration. Coupled with upper-air circulation patterns, LNOx can accumulate in significant amount in the upper troposphere with other precursors, thus enhancing ozone production (see attached figure). While LNOx emission has been included and tuned extensively in global climate models, its inclusions in regional chemistry models are seldom tested. Here we present a study that evaluates the frequently used Price and Rind parameterization based on cloud-top height at resolutions that partially resolve deep convection using the Weather Research and Forecasting model with Chemistry (WRF-Chem) over the contiguous United States. With minor modifications, the parameterization is shown to generate integrated flash counts close to those observed. However, the modeled frequency distribution of cloud-to-ground flashes do not represent well for storms with high flash rates, bringing into question the applicability of the intra-cloud/ground partitioning (IC:CG) formulation of Price and Rind in some studies. Resolution dependency also requires attention when sub-grid cloud-tops are used instead of the originally intended grid-averaged cloud-top. LNOx passive tracers being gathered by monsoonal upper tropospheric anticyclone.

  8. Viscous organic aerosol particles in the upper troposphere: diffusivity-controlled water uptake and ice nucleation?

    Directory of Open Access Journals (Sweden)

    D. M. Lienhard

    2015-12-01

    secondary organic aerosol (SOA material produced by oxidation of α-pinene and in a number of organic/inorganic model mixtures (3-methylbutane-1,2,3-tricarboxylic acid (3-MBTCA, levoglucosan, levoglucosan/NH4HSO4, raffinose are presented. These indicate that water diffusion coefficients are determined by several properties of the aerosol substance and cannot be inferred from the glass transition temperature or bouncing properties. Our results suggest that water diffusion in SOA particles is faster than often assumed and imposes no significant kinetic limitation on water uptake and release at temperatures above 220 K. The fast diffusion of water suggests that heterogeneous ice nucleation on a glassy core is very unlikely in these systems. At temperatures below 220 K, model simulations of SOA particles suggest that heterogeneous ice nucleation may occur in the immersion mode on glassy cores which remain embedded in a liquid shell when experiencing fast updraft velocities. The particles absorb significant quantities of water during these updrafts which plasticize their outer layers such that these layers equilibrate readily with the gas phase humidity before the homogeneous ice nucleation threshold is reached. Glass formation is thus unlikely to restrict homogeneous ice nucleation. Only under most extreme conditions near the very high tropical tropopause may the homogeneous ice nucleation rate coefficient be reduced as a consequence of slow condensed-phase water diffusion. Since the differences between the behavior limited or non limited by diffusion are small even at the very high tropical tropopause, condensed-phase water diffusivity is unlikely to have significant consequences on the direct climatic effects of SOA particles under tropospheric conditions.

  9. Does acetone react with HO2 in the upper-troposphere?

    Directory of Open Access Journals (Sweden)

    J. Lelieveld

    2012-02-01

    Full Text Available Recent theoretical calculations showed that reaction with HO2 could be an important sink for acetone (CH3C(OCH3 and source of acetic acid (CH3C(OOH in cold parts of the atmosphere (e.g. the tropopause region. This work details studies of HO2 + CH3C(OCH3 (CH32C(OHOO (R1 in laboratory-based and theoretical chemistry experiments; the atmospheric significance of Reaction (R1 was assessed in a global 3-D chemical model. Pulsed laser-kinetic experiments were conducted, for the first time, at the low-temperatures representative of the tropopause. Reaction with NO converted HO2 to OH for detection by laser induced fluorescence. Reduced yields of OH at T 2 by CH3C(OCH3 with a forward rate coefficient greater than 2 × 10−12 cm3 molecule−1 s−1. No evidence for Reaction (R1 was observed at T > 230 K, probably due to rapid thermal dissociation back to HO2 + CH3C(OCH3. Numerical simulations of the data indicate that these experiments were sensitive to only (R1a HO2-CH3C(OCH3 complex formation, the first step in (R1. Rearrangement (R1b of the complex to form peroxy radicals, and hence the atmospheric significance of (R1 has yet to be rigorously verified by experiment. Results from new quantum chemical calculations indicate that K1 is characterised by large uncertainties of at least an order of magnitude at T 3C(OCH3 near the tropopause, it cannot explain observations of CH3C(OOH throughout the troposphere.

  10. The influence of tropospheric static stability on upper-level frontogenesis

    OpenAIRE

    Saute, Marcel

    2011-01-01

    Upper-level frontogenesis in an inviscid, dry and adiabatic fluid forced by confluence is investigated by means of a two-dimensional semi-geostrophic model using the specific volume as an isentropic vertical coordinate. The initial conditions are specified given an analytical continuous potential vorticity field in the presence of a temperature contrast at the ground, the lower boundary condition requiring an appropriate treatment because the ground intersects the first levels of the model. T...

  11. Overview and sample applications of SMILES and Odin-SMR retrievals of upper tropospheric humidity and cloud ice mass

    Directory of Open Access Journals (Sweden)

    P. Eriksson

    2014-12-01

    Full Text Available Retrievals of cloud ice mass and humidity from the Superconducting Submillimeter-Wave Limb-Emission Sounder (SMILES and the Odin-SMR (Sub-Millimetre Radiometer limb sounder are presented and example applications of the data are given. SMILES data give an unprecedented view of the diurnal variation of cloud ice mass. Mean regional diurnal cycles are reported and compared to some global climate models. Some improvements in the models regarding diurnal timing and relative amplitude were noted, but the models' mean ice mass around 250 hPa is still low compared to the observations. The influence of the ENSO (El Niño–Southern Oscillation state on the upper troposphere is demonstrated using 12 years of Odin-SMR data. The same retrieval scheme is applied for both sensors, and gives low systematic differences between the two data sets. A special feature of this Bayesian retrieval scheme, of Monte Carlo integration type, is that values are produced for all measurements but for some atmospheric states retrieved values only reflect a priori assumptions. However, this "all-weather" capability allows a direct statistical comparison to model data, in contrast to many other satellite data sets. Another strength of the retrievals is the detailed treatment of "beam filling" that otherwise would cause large systematic biases for these passive cloud ice mass retrievals. The main retrieval inputs are spectra around 635/525 GHz from tangent altitudes below 8/9 km for SMILES/Odin-SMR, respectively. For both sensors, the data cover the upper troposphere between 30° S and 30° N. Humidity is reported as both relative humidity and volume mixing ratio. The vertical coverage of SMILES is restricted to a single layer, while Odin-SMR gives some profiling capability between 300 and 150 hPa. Ice mass is given as the partial ice water path above 260 hPa, but for Odin-SMR ice water content, estimates are also provided. Besides a smaller contrast between most dry and wet

  12. An Aircraft-Based Upper Troposphere Lower Stratosphere O3, CO, and H2O Climatology for the Northern Hemisphere

    Science.gov (United States)

    Tilmes, S.; Pan, L. L.; Hoor, P.; Atlas, E.; Avery, M. A.; Campos, T.; Christensen, L. E.; Diskin, G. S.; Gao, R.-S.; Herman, R. L.; hide

    2010-01-01

    We present a climatology of O3, CO, and H2O for the upper troposphere and lower stratosphere (UTLS), based on a large collection of high ]resolution research aircraft data taken between 1995 and 2008. To group aircraft observations with sparse horizontal coverage, the UTLS is divided into three regimes: the tropics, subtropics, and the polar region. These regimes are defined using a set of simple criteria based on tropopause height and multiple tropopause conditions. Tropopause ]referenced tracer profiles and tracer ]tracer correlations show distinct characteristics for each regime, which reflect the underlying transport processes. The UTLS climatology derived here shows many features of earlier climatologies. In addition, mixed air masses in the subtropics, identified by O3 ]CO correlations, show two characteristic modes in the tracer ]tracer space that are a result of mixed air masses in layers above and below the tropopause (TP). A thin layer of mixed air (1.2 km around the tropopause) is identified for all regions and seasons, where tracer gradients across the TP are largest. The most pronounced influence of mixing between the tropical transition layer and the subtropics was found in spring and summer in the region above 380 K potential temperature. The vertical extent of mixed air masses between UT and LS reaches up to 5 km above the TP. The tracer correlations and distributions in the UTLS derived here can serve as a reference for model and satellite data evaluation

  13. Ozone sonde cell current measurements and implications for observations of near-zero ozone concentrations in the tropical upper troposphere

    Directory of Open Access Journals (Sweden)

    H. Vömel

    2010-04-01

    Full Text Available Laboratory measurements of the Electrochemical Concentration Cell (ECC ozone sonde cell current using ozone free air as well as defined amounts of ozone reveal that background current measurements during sonde preparation are neither constant as a function of time, nor constant as a function of ozone concentration. Using a background current, measured at a defined timed after exposure to high ozone may often overestimate the real background, leading to artificially low ozone concentrations in the upper tropical troposphere, and may frequently lead to operator dependent uncertainties. Based on these laboratory measurements an improved cell current to partial pressure conversion is proposed, which removes operator dependent variability in the background reading and possible artifacts in this measurement. Data from the Central Equatorial Pacific Experiment (CEPEX have been reprocessed using the improved background treatment based on these laboratory measurements. In the reprocessed data set near-zero ozone events no longer occur. At Samoa, Fiji, Tahiti, and San Cristóbal, nearly all near-zero ozone concentrations occur in soundings with larger background currents. To a large extent, these events are no longer observed in the reprocessed data set using the improved background treatment.

  14. A Laser-Induced Fluorescence Instrument for Aircraft Measurements of Sulfur Dioxide in the Upper Troposphere and Lower Stratosphere

    Science.gov (United States)

    Rollins, Andrew W.; Thornberry, Troy D.; Ciciora, Steven J.; McLaughlin, Richard J.; Watts, Laurel A.; Hanisco, Thomas F.; Baumann, Esther; Giorgetta, Fabrizio R.; Bui, Thaopaul V.; Fahey, David W.

    2016-01-01

    This work describes the development and testing of a new instrument for in situ measurements of sulfur dioxide (SO2) on airborne platforms in the upper troposphere and lower stratosphere (UTLS). The instrument is based on the laser-induced fluorescence technique and uses the fifth harmonic of a tunable fiber-amplified semiconductor diode laser system at 1084.5 nm to excite SO2 at 216.9 nm. Sensitivity and background checks are achieved in flight by additions of SO2 calibration gas and zero air, respectively. Aircraft demonstration was performed during the NASA Volcano Plume Investigation Readiness and Gas-Phase and Aerosol Sulfur (VIRGAS) experiment, which was a series of flights using the NASA WB-57F during October 2015 based at Ellington Field and Harlingen, Texas. During these flights, the instrument successfully measured SO2 in the UTLS at background (non-volcanic) conditions with a precision of 2 ppt at 10 s and an overall uncertainty determined primarily by instrument drifts of +/- (16% + 0.9 ppt).

  15. Observed OH and HO2 concentrations in the upper troposphere inside and outside of Asian monsoon influenced air.

    Science.gov (United States)

    Marno, D. R.; Künstler, C.; Hens, K.; Tatum Ernest, C.; Broch, S.; Fuchs, H.; Martinez, M.; Bourtsoukidis, E.; Williams, J.; Holland, F.; Hofzumahaus, A.; Tomsche, L.; Fischer, H.; Klausner, T.; Schlager, H.; Eirenschmalz, L.; Stratmann, G.; Stock, P.; Ziereis, H.; Roiger, A.; Bohn, B.; Zahn, A.; Wahner, A.; Lelieveld, J.; Harder, H.

    2016-12-01

    The Asian monsoon convectively transports pollutants like volatile organic compounds (VOCs), NOx, and SO2 from the boundary layer over South Asia into the upper troposphere where they can potentially enter the stratosphere, or be dispersed globally. Therefore, it is crucial to understand the oxidizing capacity of this system regarding the rate of aerosol formation, and conversion of pollutants into compounds that have much shorter atmospheric lifetimes. OH plays a central role in this oxidation process. During the OMO-ASIA campaign in the summer of 2015, OH and HO2 were measured onboard the High Altitude Long-Range (HALO) Research Aircraft. Two laser-induced fluorescence instruments based on the fluorescence assay by gas expansion technique (LIF-FAGE) had been deployed, the AIR-LIF instrument from Forschungszentrum Jülich GmbH and the HORUS instrument from the Max Planck Institute for Chemistry, Mainz. To measure the chemical background of OH potentially produced inside the HORUS instrument from highly oxidized VOCs, atmospheric OH is scavenged by an Inlet Pre-injector (IPI) system. This was the first time an IPI system was implemented within an airborne LIF-FAGE instrument measuring OH and HO2. Throughout this campaign OH and HO2 were measured at 12 to 15km within the Asian monsoon anticyclone. These measurements have been contrasted by probing air outside the anticyclone in air masses influenced by North American emissions, and in very clean air masses originated from the southern hemisphere.

  16. Retrieval of water vapor vertical distributions in the upper troposphere and the lower stratosphere from SCIAMACHY limb measurements

    Directory of Open Access Journals (Sweden)

    A. Rozanov

    2011-05-01

    Full Text Available This study describes the retrieval of water vapor vertical distributions in the upper troposphere and lower stratosphere (UTLS altitude range from space-borne observations of the scattered solar light made in limb viewing geometry. First results using measurements from SCIAMACHY (Scanning Imaging Absorption spectroMeter for Atmospheric CHartographY aboard ENVISAT (Environmental Satellite are presented here. In previous publications, the retrieval of water vapor vertical distributions has been achieved exploiting either the emitted radiance leaving the atmosphere or the transmitted solar radiation. In this study, the scattered solar radiation is used as a new source of information on the water vapor content in the UTLS region. A recently developed retrieval algorithm utilizes the differential absorption structure of the water vapor in 1353–1410 nm spectral range and yields the water vapor content in the 11–25 km altitude range. In this study, the retrieval algorithm is successfully applied to SCIAMACHY limb measurements and the resulting water vapor profiles are compared to in situ balloon-borne observations. The results from both satellite and balloon-borne instruments are found to agree typically within 10 %.

  17. Nitric acid particles in cold thick ice clouds observed at global scale: Link with lightning, temperature, and upper tropospheric water vapor

    Science.gov (United States)

    Chepfer, H.; Minnis, P.; Dubuisson, P.; Chiriaco, M.; Sun-Mack, S.; RivièRe, E. D.

    2007-03-01

    Signatures of nitric acid particles (NAP) in cold thick ice clouds have been derived from satellite observations. Most NAP are detected in the tropics (9 to 20% of clouds with T < 202.5 K). Higher occurrences were found in the rare midlatitudes very cold clouds. NAP occurrence increases as cloud temperature decreases, and NAP are more numerous in January than July. Comparisons of NAP and lightning distributions show that lightning seems to be the main source of the NOx, which forms NAP in cold clouds over continents. Qualitative comparisons of NAP with upper tropospheric humidity distributions suggest that NAP may play a role in the dehydration of the upper troposphere when the tropopause is colder than 195 K.

  18. Review of zonal flows

    International Nuclear Information System (INIS)

    Diamond, P.H.; Itoh, S.-I.; Itoh, K.; Hahm, T.S.

    2004-10-01

    A comprehensive review of zonal flow phenomena in plasmas is presented. While the emphasis is on zonal flows in laboratory plasmas, zonal flows in nature are discussed as well. The review presents the status of theory, numerical simulation and experiments relevant to zonal flows. The emphasis is on developing an integrated understanding of the dynamics of drift wave - zonal flow turbulence by combining detailed studies of the generation of zonal flows by drift waves, the back-interaction of zonal flows on the drift waves, and the various feedback loops by which the system regulates and organizes itself. The implications of zonal flow phenomena for confinement in, and the phenomena of fusion devices are discussed. Special attention is given to the comparison of experiment with theory and to identifying direction for progress in future research. (author)

  19. MIPAS measurements of upper tropospheric C2H6 and O3 during the southern hemispheric biomass burning season in 2003

    Directory of Open Access Journals (Sweden)

    T. Steck

    2007-11-01

    Full Text Available Under cloud free conditions, the Michelson Interferometer for Passive Atmospheric Sounding (MIPAS provides measurements of spectrally resolved limb radiances down to the upper troposphere. These are used to infer global distributions of mixing ratios of atmospheric constituents in the upper troposphere and the stratosphere. From 21 October to 12 November 2003, MIPAS observed enhanced amounts of upper tropospheric C2H6 (up to about 400 pptv and ozone (up to about 80 ppbv. The absolute values of C2H6, however, may be systematically low by about 30% due to uncertainties of the spectroscopic data used. By means of trajectory calculations, the enhancements observed in the southern hemisphere are, at least partly, attributed to a biomass burning plume, which covers wide parts of the Southern hemisphere, from South America, the Atlantic Ocean, Africa, the Indian Ocean to Australia. The chemical composition of the part of the plume-like pollution belt associated with South American fires, where rainforest burning is predominant appears different from the part of the plume associated with southern African savanna burning. In particular, African savanna fires lead to a larger ozone enhancement than equatorial American fires. In this analysis, MIPAS observations of high ozone were disregarded where low CFC-11 (below 245 pptv was observed, because this hints at a stratospheric component in the measured signal. Different type of vegetation burning (flaming versus smouldering combustion has been identified as a candidate explanation for the different plume compositions.

  20. Observations of HO{sub x}, NO{sub x}, NO{sub y}, and CO. NO{sub x} control of the photochemical production and removal of ozone in the upper troposphere

    Energy Technology Data Exchange (ETDEWEB)

    Wennberg, P O; Hanisco, T F; Lanzendorf, E L; Jaegle, L Y; Jacob, D J; Cohen, R C; Anderson, J G [Harvard Univ., Cambridge, MA (United States). Dept. of Chemistry; [Dept. of Earth and Planetary Sciences; Fahey, D W; Gao, R S; Keim, E R [National Oceanic and Atmospheric Administration, Boulder, CO (United States). Aeronomy Lab.; others, and

    1998-12-31

    In-situ measurements from the NASA ER2 aircraft provide the first observations of the odd-hydrogen radicals in the upper troposphere. A new photochemical model was constructed to explain the observations. Based on the model, the way of NO{sub x} influence on the photochemistry of ozone was determined. The measurements also explain why high NO{sub x}/NO{sub y} ratios are sustained in the upper troposphere. (R.P.)

  1. Observations of HO{sub x}, NO{sub x}, NO{sub y}, and CO. NO{sub x} control of the photochemical production and removal of ozone in the upper troposphere

    Energy Technology Data Exchange (ETDEWEB)

    Wennberg, P.O.; Hanisco, T.F.; Lanzendorf, E.L.; Jaegle, L.Y.; Jacob, D.J.; Cohen, R.C.; Anderson, J.G. [Harvard Univ., Cambridge, MA (United States). Dept. of Chemistry]|[Dept. of Earth and Planetary Sciences; Fahey, D.W.; Gao, R.S.; Keim, E.R. [National Oceanic and Atmospheric Administration, Boulder, CO (United States). Aeronomy Lab.; and others

    1997-12-31

    In-situ measurements from the NASA ER2 aircraft provide the first observations of the odd-hydrogen radicals in the upper troposphere. A new photochemical model was constructed to explain the observations. Based on the model, the way of NO{sub x} influence on the photochemistry of ozone was determined. The measurements also explain why high NO{sub x}/NO{sub y} ratios are sustained in the upper troposphere. (R.P.)

  2. The effects of deep convection on the concentration and size distribution of aerosol particles within the upper troposphere: A case study

    Science.gov (United States)

    Yin, Yan; Chen, Qian; Jin, Lianji; Chen, Baojun; Zhu, Shichao; Zhang, Xiaopei

    2012-11-01

    A cloud resolving model coupled with a spectral bin microphysical scheme was used to investigate the effects of deep convection on the concentration and size distribution of aerosol particles within the upper troposphere. A deep convective storm that occurred on 1 December, 2005 in Darwin, Australia was simulated, and was compared with available radar observations. The results showed that the radar echo of the storm in the developing stage was well reproduced by the model. Sensitivity tests for aerosol layers at different altitudes were conducted in order to understand how the concentration and size distribution of aerosol particles within the upper troposphere can be influenced by the vertical transport of aerosols as a result of deep convection. The results indicated that aerosols originating from the boundary layer can be more efficiently transported upward, as compared to those from the mid-troposphere, due to significantly increased vertical velocity through the reinforced homogeneous freezing of droplets. Precipitation increased when aerosol layers were lofted at different altitudes, except for the case where an aerosol layer appeared at 5.4-8.0 km, in which relatively more efficient heterogeneous ice nucleation and subsequent Wegener-Bergeron-Findeisen process resulted in more pronounced production of ice crystals, and prohibited the formation of graupel particles via accretion. Sensitivity tests revealed, at least for the cases considered, that the concentration of aerosol particles within the upper troposphere increased by a factor of 7.71, 5.36, and 5.16, respectively, when enhanced aerosol layers existed at 0-2.2 km, 2.2-5.4 km, and 5.4-8.0 km, with Aitken mode and a portion of accumulation mode (0.1-0.2μm) particles being the most susceptible to upward transport.

  3. ATom observations of new particle formation in the tropical upper troposphere. The role of convection and nucleation mechanisms

    Science.gov (United States)

    Kupc, A.; Williamson, C.; Hodshire, A. L.; Pierce, J. R.; Ray, E. A.; Froyd, K. D.; Richardson, M.; Weinzierl, B.; Dollner, M.; Erdesz, F.; Bui, T. V.; Diskin, G. S.; Brock, C. A.

    2017-12-01

    Measurements of size distributions during the Atmospheric Tomography Mission (ATom) reveal high number concentrations (>>1000 cm-3) of nucleation mode particles at high altitudes in the tropics and subtropics under low condensation sink conditions and are associated with upwelling in convective clouds. The broad spatial extent of these newly formed particles shows that the upper free troposphere (FT) of the tropics and subtropics is a globally significant source. In this study, we investigate the link between convection and new particle formation (NPF) by exploring the processes that govern NPF and growth in the tropical and subtropical FT of the Pacific and Atlantic Oceans. We use measurements of the size distributions made with a suite of fast-response instruments on board of a NASA DC-8 aircraft during ATom mission. ATom maps the remote atmosphere over the Pacific and Atlantic basins ( 80 °N and 65 °S) in continuous ascents and descents (0.2 and 13 km), providing the latitudinal and vertical information on the greenhouse gases, reactive and tracer species and aerosol properties and their seasonal variability. We couple measurements of size distributions between 0.003 and 4.8 µm and potential aerosol precursor vapors measured on ATom (August 2016 and February 2017) with calculated air mass back trajectories and the TwO-Moment Aerosol Sectional (TOMAS) box model. The back trajectories identify air masses potentially influenced by recent convection. We then use TOMAS to model particle nucleation, condensation and coagulation along that trajectory to investigate the link between convection and NPF. Through TOMAS, we explore the influence of different nucleation mechanisms (such as binary, ternary or the one with organics) and gas-phase aerosol precursors (such as sulfur dioxide) on observed particle size distributions. We discuss similarities and differences in NPF over the Pacific and Atlantic Oceans and their relationship to convection, examine particle

  4. Observations of fine-scale transport structure in the upper troposphere from the High-performance Instrumented Airborne Platform for Environmental Research

    Science.gov (United States)

    Bowman, Kenneth P.; Pan, Laura L.; Campos, Teresa; Gao, Rushan

    2007-09-01

    The Progressive Science Mission in December 2005 was the first research use of the new NCAR High-performance Instrumented Airborne Platform for Environmental Research (HIAPER) aircraft. The Stratosphere-Troposphere Analyses of Regional Transport (START) component of the mission was designed to investigate the dynamical and chemical structure of the upper troposphere and lower stratosphere. Flight 5 of the Progressive Science mission was a START flight that sampled near the tropopause in an area between the main jet stream and a large, quasi-stationary, cutoff low. The large-scale flow in this region was characterized by a hyperbolic (saddle) point. In this study the in situ measurements by HIAPER are combined with flow analyses and satellite data to investigate the quasi-isentropic stirring of trace species in the upper troposphere. As expected from theoretical considerations, strong stretching and folding deformation of the flow near the hyperbolic point resulted in rapid filamentation of air masses and sharp gradients of constituents. Calculations of the stirring using operational meteorological analyses from the NCEP Global Forecast System model produced excellent agreement with HIAPER and satellite observations of trace species. Back trajectories indicate that elevated ozone levels in some filaments likely came from a large stratospheric intrusion that occurred upstream in the jet over the north Pacific Ocean. The methods presented here can be used with operational forecasts for future flight planning.

  5. The 4-5 day mode oscillation in zonal winds of Indian middle atmosphere during MONEX-79

    Science.gov (United States)

    Reddy, R. S.; Mukherjee, B. K.; Indira, K.; Murty, B. V. R.

    1985-12-01

    In the early studies based on time series of balloon observations, the existence of 4 to 5 day period waves and 10 to 20 day wind fluctuations were found in the tropical lower stratosphere, and they are identified theoretically as the mixed Rossby-gravity wave and the Kelvin wave, respectively. On the basis of these studies, it was established that the vertically propagating equatorial waves play an important role in producing the QBO (quasi-biennial oscillation) in the mean zonal wind through the mechanism of wave-zonal interaction. These studies are mainly concentrated over the equatorial Pacific and Atlantic Oceans. Similar prominent wave disturbances have been observed over the region east of the Indian Ocean during a quasi-biennial oscillation. Zonal winds in upper troposphere and lower stratosphere (10 to 20) km of the middle atmosphere over the Indian subcontinent may bear association with the activity of summer monsoon (June-September). Monsoon Experiment (MONEX-79) has provided upper air observations at Balasore (21 deg. 30 min.N; 85 deg. 56 min.E), during the peak of monsoon months July and August. A unique opportunity has, therefore, been provided to study the normal oscillations present in the zonal winds of lower middle atmosphere over India, which may have implication on large scale wave dynamics. This aspect is examined in the present study.

  6. Transport of Formaldehyde to the Upper Troposphere In Deep Convective Storms During the 2012 DC3 Study

    Science.gov (United States)

    Fried, A.; Weibring, P.; Richter, D.; Walega, J.; Olson, J. R.; Crawford, J. H.; Barth, M. C.; Apel, E. C.; Hornbrook, R. S.; Bela, M. M.; Toon, O. B.; Blake, D. R.; Blake, N. J.; Luo, Z. J.

    2014-12-01

    The Deep Convective Clouds and Chemistry (DC3) campaign in the summer of 2012 provided an opportunity to study the impacts of deep convection on reactive and soluble precursors of ozone and HOx radicals, including CH2O, in the upper troposphere and lower stratosphere (UTLS) over North America. Formaldehyde measurements were acquired in the inflow and outflow of numerous storms on the NASA DC-8 and NSF/NCAR GV-aircraft employing fast, sensitive, and accurate difference frequency generation infrared absorption spectrometers. Since our Fall 2013 AGU Meeting poster, we have developed an improved methodology based upon 3 independent approaches, to determine the amount of CH2O that is scavenged by deep convective storms. The first approach is based upon WRF-Chem model simulations, which provides greater confidence in the determination of CH2O scavenging efficiencies and allows the estimation of CH2O ice retention factors.The second approach is a modified mixing model employing 4 non-reactive passive tracers (n,i-butane, n,i-pentane) to estimate altitude-dependent lateral entrainment rates. This information is coupled with time-dependent measurements in the outflow of various storms, which when extrapolated to time zero in the storm core, results in estimates of CH2O scavenging efficiencies. This analysis includes estimates of photochemically produced CH2O in the storm core. A third approach is based upon CH2O/n-butane ratio comparisons in both the storm inflow and outflow. Results from various storms over Oklahoma, Colorado, and Alabama will be presented. However, the analysis will primarily focus on the May 29, 2012 supercell storm in Oklahoma. During this storm, the 4 passive tracers produced a very consistent lateral entrainment rate of 0.083 ± 0.008 km-1, a value that broadly agrees with entrainment rates determined previously from analyzing moist static energy profiles (Luo et al., Geophys. Res. Lett., 2010). For this storm, the 3-independent approaches give CH2O

  7. Physics of zonal flows

    International Nuclear Information System (INIS)

    Itoh, K.; Fujisawa, A.; Itoh, S.-I.; Yagi, M.; Nagashima, Y.; Diamond, P.H.; Tynan, G.R.; Hahm, T.S.

    2006-01-01

    Zonal flows, which means azimuthally symmetric band-like shear flows, are ubiquitous phenomena in nature and the laboratory. It is now widely recognized that zonal flows are a key constituent in virtually all cases and regimes of drift wave turbulence, indeed, so much so that this classic problem is now frequently referred to as ''drift wave-zonal flow turbulence.'' In this review, new viewpoints and unifying concepts are presented, which facilitate understanding of zonal flow physics, via theory, computation and their confrontation with the results of laboratory experiment. Special emphasis is placed on identifying avenues for further progress. (author)

  8. Physics of zonal flows

    International Nuclear Information System (INIS)

    Itoh, K.; Itoh, S.-I.; Diamond, P.H.; Hahm, T.S.; Fujisawa, A.; Tynan, G.R.; Yagi, M.; Nagashima, Y.

    2006-01-01

    Zonal flows, which means azimuthally symmetric band-like shear flows, are ubiquitous phenomena in nature and the laboratory. It is now widely recognized that zonal flows are a key constituent in virtually all cases and regimes of drift wave turbulence, indeed, so much so that this classic problem is now frequently referred to as 'drift wave-zonal flow turbulence'. In this review, new viewpoints and unifying concepts are presented, which facilitate understanding of zonal flow physics, via theory, computation and their confrontation with the results of laboratory experiment. Special emphasis is placed on identifying avenues for further progress

  9. Interrelated variations of O3, CO and deep convection in the tropical/subtropical upper troposphere observed by the Aura Microwave Limb Sounder (MLS during 2004–2011

    Directory of Open Access Journals (Sweden)

    L. Froidevaux

    2013-01-01

    Full Text Available The interrelated geographic and temporal variability seen in more than seven years of tropical and subtropical upper tropospheric (215 hPa ozone, carbon monoxide and cloud ice water content (IWC observations by the Aura Microwave Limb Sounder (MLS are presented. Observed ozone abundances and their variability (geographic and temporal agree to within 10–15 ppbv with records from sonde observations. MLS complements these (and other observations with global coverage and simultaneous measurements of related parameters. Previously-reported phenomena such as the ozone "wave one" feature are clearly seen in the MLS observations, as is a double peak in ozone abundance over tropical East Africa, with enhanced abundances in both May to June and September to November. While repeatable seasonal cycles are seen in many regions, they are often accompanied by significant interannual variability. Ozone seasonal cycles in the southern tropics and subtropics tend to be more distinct (i.e., annually repeatable than in the northern. By contrast, carbon monoxide shows distinct seasonal cycles in many northern subtropical regions, notably from India to the Eastern Pacific. Deep convection (as indicated by large values of IWC is typically associated with reductions in upper tropospheric ozone. Convection over polluted regions is seen to significantly enhance upper tropospheric carbon monoxide. While some regions show statistically significant correlations among ozone, carbon monoxide and IWC, simple correlations fall well short of accounting for the observed variability. The observed interrelated variations and metrics of annual and interannual variability described here represent a new resource for validation of atmospheric chemistry models.

  10. The Vertical Structure of Relative Humidity and Ozone in the Tropical Upper Troposphere: Intercomparisons Among In Situ Observations, A-Train Measurements and Large-Scale Models

    Science.gov (United States)

    Selkirk, Henry B.; Manyin, Michael; Douglass, Anne R.; Oman, Luke; Pawson, Steven; Ott, Lesley; Benson, Craig; Stolarski, Richard

    2010-01-01

    In situ measurements in the tropics have shown that in regions of active convection, relative humidity with respect to ice in the upper troposphere is typically close to saturation on average, and supersaturations greater than 20% are not uncommon. Balloon soundings with the cryogenic frost point hygrometer (CFH) at Costa Rica during northern summer, for example, show this tendency to be strongest between 11 and 15.5 km (345-360 K potential temperature, or approximately 250-120 hPa). this is the altitude range of deep convective detrainment. Additionally, simultaneous ozonesonde measurements show that stratospheric air (O3 greater than 150 ppbv) can be found as low as approximately 14 km (350 K/150 hPa). In contrast, results from northern winter show a much drier upper troposphere and little penetration of stratospheric air below the tropopause at 17.5 km (approximately 383 K). We show that these results are consistent with in situ measurements from the Measurement of Ozone and water vapor by Airbus In-service airCraft (MOZAIC) program which samples a wider, though still limited, range of tropical locations. To generalize to the tropics as a whole, we compare our insitu results to data from two A-Train satellite instruments, the Atmospheric Infrared Sounder (AIRS) and the Microwave Limb Sounder (MLS) on the Aqua and Aura satellites respectively. Finally, we examine the vertical structure of water vapor, relative humidity and ozone in the NASA Goddard MERRA analysis, an assimilation dataset, and a new version of the GEOS CCM, a free-running chemistry-climate model. We demonstrate that conditional probability distributions of relative humidity and ozone are a sensitive diagnostic for assessing the representation of deep convection and upper troposphere/lower stratosphere mixing processes in large-scale analyses and climate models.

  11. Inertia gravity waves in the upper troposphere during the MaCWAVE winter campaign – Part I: Observations with collocated radars

    Directory of Open Access Journals (Sweden)

    P. Hoffmann

    2006-11-01

    Full Text Available During the {MaCWAVE} campaign, combined rocket, radiosonde and ground-based measurements have been performed at the Norwegian Andøya Rocket Range (ARR near Andenes and the Swedish Rocket Range (ESRANGE near Kiruna in January 2003 to study gravity waves in the vicinity of the Scandinavian mountain ridge. The investigations presented here are mainly based on the evaluation of continuous radar measurements with the ALWIN VHF radar in the upper troposphere/ lower stratosphere at Andenes (69.3° N, 16.0° E and the ESRAD VHF radar near Kiruna (67.9° N, 21.9° E. Both radars are separated by about 260 km. Based on wavelet transformations of both data sets, the strongest activity of inertia gravity waves in the upper troposphere has been detected during the first period from 24–26 January 2003 with dominant vertical wavelengths of about 4–5 km as well as with dominant observed periods of about 13–14 h for the altitude range between 5 and 8 km under the additional influence of mountain waves. The results show the appearance of dominating inertia gravity waves with characteristic horizontal wavelengths of ~200 km moving in the opposite direction than the mean background wind. The results show the appearance of dominating inertia gravity waves with intrinsic periods in the order of ~5 h and with horizontal wavelengths of 200 km, moving in the opposite direction than the mean background wind. From the derived downward energy propagation it is supposed, that these waves are likely generated by a jet streak in the upper troposphere. The parameters of the jet-induced gravity waves have been estimated at both sites separately. The identified gravity waves are coherent at both locations and show higher amplitudes on the east-side of the Scandinavian mountain ridge, as expected by the influence of mountains.

  12. Correction Technique for Raman Water Vapor Lidar Signal-Dependent Bias and Suitability for Water Wapor Trend Monitoring in the Upper Troposphere

    Science.gov (United States)

    Whiteman, D. N.; Cadirola, M.; Venable, D.; Calhoun, M.; Miloshevich, L; Vermeesch, K.; Twigg, L.; Dirisu, A.; Hurst, D.; Hall, E.; hide

    2012-01-01

    The MOHAVE-2009 campaign brought together diverse instrumentation for measuring atmospheric water vapor. We report on the participation of the ALVICE (Atmospheric Laboratory for Validation, Interagency Collaboration and Education) mobile laboratory in the MOHAVE-2009 campaign. In appendices we also report on the performance of the corrected Vaisala RS92 radiosonde measurements during the campaign, on a new radiosonde based calibration algorithm that reduces the influence of atmospheric variability on the derived calibration constant, and on other results of the ALVICE deployment. The MOHAVE-2009 campaign permitted the Raman lidar systems participating to discover and address measurement biases in the upper troposphere and lower stratosphere. The ALVICE lidar system was found to possess a wet bias which was attributed to fluorescence of insect material that was deposited on the telescope early in the mission. Other sources of wet biases are discussed and data from other Raman lidar systems are investigated, revealing that wet biases in upper tropospheric (UT) and lower stratospheric (LS) water vapor measurements appear to be quite common in Raman lidar systems. Lower stratospheric climatology of water vapor is investigated both as a means to check for the existence of these wet biases in Raman lidar data and as a source of correction for the bias. A correction technique is derived and applied to the ALVICE lidar water vapor profiles. Good agreement is found between corrected ALVICE lidar measurments and those of RS92, frost point hygrometer and total column water. The correction is offered as a general method to both quality control Raman water vapor lidar data and to correct those data that have signal-dependent bias. The influence of the correction is shown to be small at regions in the upper troposphere where recent work indicates detection of trends in atmospheric water vapor may be most robust. The correction shown here holds promise for permitting useful upper

  13. Model Calculations of Changes in Tropospheric Ozone Over Europe and the Role of Surface Sources and Aircraft Emissions

    Energy Technology Data Exchange (ETDEWEB)

    Hov, Oe [Bergen Univ. (Norway)

    1996-01-01

    This conference paper deals with a study of the impact of various sources of NO{sub x} on the ozone production in the free troposphere. A comprehensive two-dimensional zonally averaged chemistry/transport model and a three-dimensional meso-scale chemical transport (MCT) model are used in the study. Using the two-dimensional model, three surches of NO{sub x} in the upper troposphere were examined covering NO{sub x} produced by lightening, NO{sub x} (and NO{sub y}) brought to the upper troposphere from the planetary boundary layer by rapid vertical transport processes, and NO{sub x} emitted from aircraft. 4 refs.

  14. Inertia gravity waves in the upper troposphere during the MaCWAVE winter campaign. Part II. Radar investigations and modelling studies

    Energy Technology Data Exchange (ETDEWEB)

    Serafimovich, A.; Zuelicke, C.; Hoffmann, P.; Peters, D.; Singer, W. [Leibniz-Inst. fuer Atmosphaerenphysik, Kuehlungsborn (Germany); Dalin, P. [Swedish Inst. of Space Physics, Kiruna (Sweden)

    2006-07-01

    We present an experimental and modelling study of a strong gravity wave event in the upper troposphere/lower stratosphere near the Scandinavian mountain ridge. Continuous VHP radar measurements during the MaCWAVE rocket and ground-based measurement campaign were performed at the Norwegian Andoya rocket range (ARR) near Andenes (69.3 N, 16 E) in January 2003. Detailed gravity wave investigations based on PSU/NCAR fifth-generation mesoscale model (MM5) data have been used for comparison with experimentally obtained results. The model data show the presence of a mountain wave and of an inertia gravity wave generated by a jet streak near the tropopause region. Temporal and spatial dependencies of jet induced inertia gravity waves with dominant observed periods of about 13 h and vertical wavelengths of {proportional_to}4.5-5 km are investigated with wavelet transform applied on radar measurements and model data. The jet induced wave packet is observed to move upstream and downward in the upper troposphere. The model data agree with the experimentally obtained results fairly well. Possible reasons for the observed differences, e.g. in the time of maximum of the wave activity, are discussed. Finally, the vertical fluxes of horizontal momentum are estimated with different methods and provide similar amplitudes. We found indications that the derived positive vertical flux of the horizontal momentum corresponds to the obtained parameters of the jet-induced inertia gravity wave, but only at the periods and heights of the strongest wave activity. (orig.)

  15. Potential impact of carbonaceous aerosol on the upper troposphere and lower stratosphere (UTLS) and precipitation during Asian summer monsoon in a global model simulation

    KAUST Repository

    Fadnavis, Suvarna

    2017-09-28

    Recent satellite observations show efficient vertical transport of Asian pollutants from the surface to the upper-level anticyclone by deep monsoon convection. In this paper, we examine the transport of carbonaceous aerosols, including black carbon (BC) and organic carbon (OC), into the monsoon anticyclone using of ECHAM6-HAM, a global aerosol climate model. Further, we investigate impacts of enhanced (doubled) carbonaceous aerosol emissions on the upper troposphere and lower stratosphere (UTLS), underneath monsoon circulation and precipitation from sensitivity simulations. The model simulation shows that boundary layer aerosols are transported into the monsoon anticyclone by the strong monsoon convection from the Bay of Bengal, southern slopes of the Himalayas and the South China Sea. Doubling of emissions of both BC and OC aerosols over Southeast Asia (10° S–50° N, 65–155° E) shows that lofted aerosols produce significant warming (0.6–1 K) over the Tibetan Plateau (TP) near 400–200 hPa and instability in the middle/upper troposphere. These aerosols enhance radiative heating rates (0.02–0.03 K day−1) near the tropopause. The enhanced carbonaceous aerosols alter aerosol radiative forcing (RF) at the surface by −4.74 ± 1.42 W m−2, at the top of the atmosphere (TOA) by +0.37 ± 0.26 W m−2 and in the atmosphere by +5.11 ± 0.83 W m−2 over the TP and Indo-Gangetic Plain region (15–35° N, 80–110° E). Atmospheric warming increases vertical velocities and thereby cloud ice in the upper troposphere. Aerosol induced anomalous warming over the TP facilitates the relative strengthening of the monsoon Hadley circulation and increases moisture inflow by strengthening the cross-equatorial monsoon jet. This increases precipitation amounts over India (1–4 mm day−1) and eastern China (0.2–2 mm day−1). These results are significant at the 99 % confidence level.

  16. Continental outflow from the US to the upper troposphere over the North Atlantic during the NASA INTEX-NA Airborne Campaign

    Directory of Open Access Journals (Sweden)

    S. Y. Kim

    2008-04-01

    Full Text Available A case of continental outflow from the United States (US was examined using airborne measurements from NASA DC-8 flight 13 during the Intercontinental Chemical Transport Experiment – North America (INTEX-NA. Mixing ratios of methane (CH4 and carbon monoxide (CO at 8–11 km altitude over the North Atlantic were elevated to 1843 ppbv and 134 ppbv respectively, while those of carbon dioxide (CO2 and carbonyl sulfide (COS were reduced to 372.4 ppmv and 411 pptv respectively. In this region, urban and industrial influences were evidenced by elevated mixing ratios and good linear relationships between urban and industrial tracers compared to North Atlantic background air. Moreover, low mixing ratios and a good correlation between COS and CO2 showed a fingerprint of terrestrial uptake and minimal dilution during rapid transport over a 1–2 day time period. Analysis of synoptic conditions, backward trajectories, and photochemical aging estimates based on C3H8/C2H6 strongly suggested that elevated anthropogenic tracers in the upper troposphere of the flight region were the result of transport via convection and warm conveyor belt (WCB uplifting of boundary layer air over the southeastern US. This mechanism is supported by the similar slope values of linear correlations between long-lived (months anthropogenic tracers (e.g., C2Cl4 and CHCl3 from the flight region and the planetary boundary layer in the southeastern US. In addition, the aircraft measurements suggest that outflow from the US augmented the entire tropospheric column at mid-latitudes over the North Atlantic. Overall, the flight 13 data demonstrate a pervasive impact of US anthropogenic emissions on the troposphere over the North Atlantic.

  17. First airborne water vapor lidar measurements in the tropical upper troposphere and mid-latitudes lower stratosphere: accuracy evaluation and intercomparisons with other instruments

    Directory of Open Access Journals (Sweden)

    C. Schiller

    2008-09-01

    Full Text Available In the tropics, deep convection is the major source of uncertainty in water vapor transport to the upper troposphere and into the stratosphere. Although accurate measurements in this region would be of first order importance to better understand the processes that govern stratospheric water vapor concentrations and trends in the context of a changing climate, they are sparse because of instrumental shortcomings and observational challenges. Therefore, the Falcon research aircraft of the Deutsches Zentrum für Luft- und Raumfahrt (DLR flew a zenith-viewing water vapor differential absorption lidar (DIAL during the Tropical Convection, Cirrus and Nitrogen Oxides Experiment (TROCCINOX in 2004 and 2005 in Brazil. The measurements were performed alternatively on three water vapor absorption lines of different strength around 940 nm. These are the first aircraft DIAL measurements in the tropical upper troposphere and in the mid-latitudes lower stratosphere. Sensitivity analyses reveal an accuracy of 5% between altitudes of 8 and 16 km. This is confirmed by intercomparisons with the Fast In-situ Stratospheric Hygrometer (FISH and the Fluorescent Advanced Stratospheric Hygrometer (FLASH onboard the Russian M-55 Geophysica research aircraft during five coordinated flights. The average relative differences between FISH and DIAL amount to −3%±8% and between FLASH and DIAL to −8%±14%, negative meaning DIAL is more humid. The average distance between the probed air masses was 129 km. The DIAL is found to have no altitude- or latitude-dependent bias. A comparison with the balloon ascent of a laser absorption spectrometer gives an average difference of 0%±19% at a distance of 75 km. Six tropical DIAL under-flights of the Michelson Interferometer for Passive Atmospheric Sounding (MIPAS on board ENVISAT reveal a mean difference of −8%±49% at an average distance of 315 km. While the comparison with MIPAS is somewhat less significant due to poorer

  18. The chemical effects on the summertime ozone in the upper troposphere and lower stratosphere over the Tibetan Plateau and the South Asian monsoon region

    Science.gov (United States)

    Gu, Yixuan; Liao, Hong; Xu, Jianming; Zhou, Guangqiang

    2018-01-01

    We use the global three-dimensional Goddard Earth Observing System chemical transport model with the Universal tropospheric-stratospheric Chemistry eXtension mechanism to examine the contributions of the chemical processes to summertime O3 in the upper troposphere and lower stratosphere (UTLS) over the Tibetan Plateau and the South Asian monsoon region (TP/SASM). Simulated UTLS O3 concentrations are evaluated by comparisons with Microwave Limb Sounder products and net chemical production of O3 (NPO3) are evaluated by comparisons with model results in previous studies. Simulations show that the chemical processes lead to an increase in O3 concentration, which is opposite to the effect of O3 transport in the UTLS over the TP/SASM region throughout the boreal summer. NPO3 in UTLS over the TP/SASM region is the largest in summer. Elevated values (0.016-0.020 Tg year-1) of the seasonal mean NPO3 are simulated to locate at 100 hPa in the TP/SASM region, where the mixing ratios of O3 are low and those of O3 precursors (NO x , VOCs, and CO) are high. The high concentrations of O3 precursors (NO x , VOCs, and CO) together with the active photochemical reactions of NO2 in the UTLS over the TP/SASM region during summertime could be important reasons for the enhancement of {NP}_{{{O}3 }} over the studied region.

  19. Potential impact of carbonaceous aerosol on the upper troposphere and lower stratosphere (UTLS) and precipitation during Asian summer monsoon in a global model simulation

    KAUST Repository

    Fadnavis, Suvarna; Kalita, Gayatry; Kumar, K. Ravi; Gasparini, Blaž; Li, Jui-Lin Frank

    2017-01-01

    The model simulation shows that boundary layer aerosols are transported into the monsoon anticyclone by the strong monsoon convection from the Bay of Bengal, southern slopes of the Himalayas and the South China Sea. Doubling of emissions of both BC and OC aerosols over Southeast Asia (10° S–50° N, 65–155° E) shows that lofted aerosols produce significant warming (0.6–1 K) over the Tibetan Plateau (TP) near 400–200 hPa and instability in the middle/upper troposphere. These aerosols enhance radiative heating rates (0.02–0.03 K day−1) near the tropopause. The enhanced carbonaceous aerosols alter aerosol radiative forcing (RF) at the surface by −4.74 ± 1.42 W m−2, at the top of the atmosphere (TOA) by +0.37 ± 0.26 W m−2 and in the atmosphere by +5.11 ± 0.83 W m−2 over the TP and Indo-Gangetic Plain region (15–35° N, 80–110° E). Atmospheric warming increases vertical velocities and thereby cloud ice in the upper troposphere. Aerosol induced anomalous warming over the TP facilitates the relative strengthening of the monsoon Hadley circulation and increases moisture inflow by strengthening the cross-equatorial monsoon jet. This increases precipitation amounts over India (1–4 mm day−1) and eastern China (0.2–2 mm day−1). These results are significant at the 99 % confidence level.

  20. NASA Goddard Earth Sciences Graduate Student Program. [FIRE CIRRUS-II examination of coupling between an upper tropospheric cloud system and synoptic-scale dynamics

    Science.gov (United States)

    Ackerman, Thomas P.

    1994-01-01

    The evolution of synoptic-scale dynamics associated with a middle and upper tropospheric cloud event that occurred on 26 November 1991 is examined. The case under consideration occurred during the FIRE CIRRUS-II Intensive Field Observing Period held in Coffeyville, KS during Nov. and Dec., 1991. Using data from the wind profiler demonstration network and a temporally and spatially augmented radiosonde array, emphasis is given to explaining the evolution of the kinematically-derived ageostrophic vertical circulations and correlating the circulation with the forcing of an extensively sampled cloud field. This is facilitated by decomposing the horizontal divergence into its component parts through a natural coordinate representation of the flow. Ageostrophic vertical circulations are inferred and compared to the circulation forcing arising from geostrophic confluence and shearing deformation derived from the Sawyer-Eliassen Equation. It is found that a thermodynamically indirect vertical circulation existed in association with a jet streak exit region. The circulation was displaced to the cyclonic side of the jet axis due to the orientation of the jet exit between a deepening diffluent trough and building ridge. The cloud line formed in the ascending branch of the vertical circulation with the most concentrated cloud development occurring in conjunction with the maximum large-scale vertical motion. The relationship between the large scale dynamics and the parameterization of middle and upper tropospheric clouds in large-scale models is discussed and an example of ice water contents derived from a parameterization forced by the diagnosed vertical motions and observed water vapor contents is presented.

  1. Inertia gravity waves in the upper troposphere during the MaCWAVE winter campaign – Part II: Radar investigations and modelling studies

    Directory of Open Access Journals (Sweden)

    A. Serafimovich

    2006-11-01

    Full Text Available We present an experimental and modelling study of a strong gravity wave event in the upper troposphere/lower stratosphere near the Scandinavian mountain ridge. Continuous VHF radar measurements during the MaCWAVE rocket and ground-based measurement campaign were performed at the Norwegian Andoya Rocket Range (ARR near Andenes (69.3° N, 16° E in January 2003. Detailed gravity wave investigations based on PSU/NCAR Fifth-Generation Mesoscale Model (MM5 data have been used for comparison with experimentally obtained results. The model data show the presence of a mountain wave and of an inertia gravity wave generated by a jet streak near the tropopause region. Temporal and spatial dependencies of jet induced inertia gravity waves with dominant observed periods of about 13 h and vertical wavelengths of ~4.5–5 km are investigated with wavelet transform applied on radar measurements and model data. The jet induced wave packet is observed to move upstream and downward in the upper troposphere. The model data agree with the experimentally obtained results fairly well. Possible reasons for the observed differences, e.g. in the time of maximum of the wave activity, are discussed. Finally, the vertical fluxes of horizontal momentum are estimated with different methods and provide similar amplitudes. We found indications that the derived positive vertical flux of the horizontal momentum corresponds to the obtained parameters of the jet-induced inertia gravity wave, but only at the periods and heights of the strongest wave activity.

  2. Investigation of inertia-gravity waves in the upper troposphere/lower stratosphere over Northern Germany observed with collocated VHF/UHF radars

    Directory of Open Access Journals (Sweden)

    A. Serafimovich

    2005-01-01

    Full Text Available A case study to investigate the properties of inertia-gravity waves in the upper troposphere/lower stratosphere has been carried out over Northern Germany during the occurrence of an upper tropospheric jet in connection with a poleward Rossby wave breaking event from 17-19 December 1999. The investigations are based on the evaluation of continuous radar measurements with the OSWIN VHF radar at Kühlungsborn (54.1 N, 11.8 E and the 482 MHz UHF wind profiler at Lindenberg (52.2 N, 14.1 E. Both radars are separated by about 265 km. Based on wavelet transformations of both data sets, the dominant vertical wavelengths of about 2-4 km for fixed times as well as the dominant observed periods of about 11 h and weaker oscillations with periods of  6 h for the altitude range between 5 and 8 km are comparable. Gravity wave parameters have been estimated at both locations separately and by a complex cross-spectral analysis of the data of both radars. The results show the appearance of dominating inertia-gravity waves with characteristic horizontal wavelengths of  300 km moving in the opposite direction than the mean background wind and a secondary less pronounced wave with a horizontal wavelength in the order of about 200 km moving with the wind. Temporal and spatial differences of the observed waves are discussed.

  3. Mercury Plumes in the Global Upper Troposphere Observed during Flights with the CARIBIC Observatory from May 2005 until June 2013

    Directory of Open Access Journals (Sweden)

    Franz Slemr

    2014-05-01

    Full Text Available Tropospheric sections of flights with the CARIBIC (Civil Aircraft for Regular Investigation of the Atmosphere Based on an Instrumented Container observatory from May 2005 until June 2013, are investigated for the occurrence of plumes with elevated Hg concentrations. Additional information on CO, CO2, CH4, NOy, O3, hydrocarbons, halocarbons, acetone and acetonitrile enable us to attribute the plumes to biomass burning, urban/industrial sources or a mixture of both. Altogether, 98 pollution plumes with elevated Hg concentrations and CO mixing ratios were encountered, and the Hg/CO emission ratios for 49 of them could be calculated. Most of the plumes were found over East Asia, in the African equatorial region, over South America and over Pakistan and India. The plumes encountered over equatorial Africa and over South America originate predominantly from biomass burning, as evidenced by the low Hg/CO emission ratios and elevated mixing ratios of acetonitrile, CH3Cl and particle concentrations. The backward trajectories point to the regions around the Rift Valley and the Amazon Basin, with its outskirts, as the source areas. The plumes encountered over East Asia and over Pakistan and India are predominantly of urban/industrial origin, sometimes mixed with products of biomass/biofuel burning. Backward trajectories point mostly to source areas in China and northern India. The Hg/CO2 and Hg/CH4 emission ratios for several plumes are also presented and discussed.

  4. Methane from the Tropospheric Emission Spectrometer (TES)

    Science.gov (United States)

    Payne, Vivienne; Worden, John; Kulawik, Susan; Frankenberg, Christian; Bowman, Kevin; Wecht, Kevin

    2012-01-01

    TES V5 CH4 captures latitudinal gradients, regional variability and interannual variation in the free troposphere. V5 joint retrievals offer improved sensitivity to lower troposphere. Time series extends from 2004 to present. V5 reprocessing in progress. Upper tropospheric bias. Mitigated by N2O correction. Appears largely spatially uniform, so can be corrected. How to relate free-tropospheric values to surface emissions.

  5. The vertical structure of Jupiter and Saturn zonal winds from nonlinear simulations of major vortices and planetary-scale disturbances

    Science.gov (United States)

    Garcia-Melendo, E.; Legarreta, J.; Sanchez-Lavega, A.

    2012-12-01

    Direct measurements of the structure of the zonal winds of Jupiter and Saturn below the upper cloud layer are very difficult to retrieve. Except from the vertical profile at a Jupiter hot spot obtained from the Galileo probe in 1995 and measurements from cloud tracking by Cassini instruments just below the upper cloud, no other data are available. We present here our inferences of the vertical structure of Jupiter and Saturn zonal wind across the upper troposphere (deep down to about 10 bar level) obtained from nonlinear simulations using the EPIC code of the stability and interactions of large-scale vortices and planetary-scale disturbances in both planets. Acknowledgements: This work has been funded by Spanish MICIIN AYA2009-10701 with FEDER support, Grupos Gobierno Vasco IT-464-07 and UPV/EHU UFI11/55. [1] García-Melendo E., Sánchez-Lavega A., Dowling T.., Icarus, 176, 272-282 (2005). [2] García-Melendo E., Sánchez-Lavega A., Hueso R., Icarus, 191, 665-677 (2007). [3] Sánchez-Lavega A., et al., Nature, 451, 437- 440 (2008). [4] Sánchez-Lavega A., et al., Nature, 475, 71-74 (2011).

  6. Spatial Heterodyne Observations of Water (SHOW) vapour in the upper troposphere and lower stratosphere from a high altitude aircraft: Modelling and sensitivity analysis

    Science.gov (United States)

    Langille, J. A.; Letros, D.; Zawada, D.; Bourassa, A.; Degenstein, D.; Solheim, B.

    2018-04-01

    A spatial heterodyne spectrometer (SHS) has been developed to measure the vertical distribution of water vapour in the upper troposphere and the lower stratosphere with a high vertical resolution (∼500 m). The Spatial Heterodyne Observations of Water (SHOW) instrument combines an imaging system with a monolithic field-widened SHS to observe limb scattered sunlight in a vibrational band of water (1363 nm-1366 nm). The instrument has been optimized for observations from NASA's ER-2 aircraft as a proof-of-concept for a future low earth orbit satellite deployment. A robust model has been developed to simulate SHOW ER-2 limb measurements and retrievals. This paper presents the simulation of the SHOW ER-2 limb measurements along a hypothetical flight track and examines the sensitivity of the measurement and retrieval approach. Water vapour fields from an Environment and Climate Change Canada forecast model are used to represent realistic spatial variability along the flight path. High spectral resolution limb scattered radiances are simulated using the SASKTRAN radiative transfer model. It is shown that the SHOW instrument onboard the ER-2 is capable of resolving the water vapour variability in the UTLS from approximately 12 km - 18 km with ±1 ppm accuracy. Vertical resolutions between 500 m and 1 km are feasible. The along track sampling capability of the instrument is also discussed.

  7. On the long-term variability of Jupiter and Saturn zonal winds

    Science.gov (United States)

    Sanchez-Lavega, A.; Garcia-Melendo, E.; Hueso, R.; Barrado-Izagirre, N.; Legarreta, J.; Rojas, J. F.

    2012-12-01

    We present an analysis of the long-term variability of Jupiter and Saturn zonal wind profiles at their upper cloud level as retrieved from cloud motion tracking on images obtained at ground-based observatories and with different spacecraft missions since 1979, encompassing about three Jovian and one Saturn years. We study the sensitivity and variability of the zonal wind profile in both planets to major planetary-scale disturbances and to seasonal forcing. We finally discuss the implications that these results have for current model efforts to explain the global tropospheric circulation in these planets. Acknowledgements: This work has been funded by Spanish MICIIN AYA2009-10701 with FEDER support, Grupos Gobierno Vasco IT-464-07 and UPV/EHU UFI11/55. [1] Sánchez-Lavega A., et al., Icarus, 147, 405-420 (2000). [2] García-Melendo E., Sánchez LavegaA., Icarus, 152, 316-330 (2001) [3] Sánchez-Lavega A., et al., Nature, 423, 623-625 (2003). [4] García-Melendo E., et al., Geophysical Research Letters, 37, L22204 (2010).

  8. Complex chemical composition of colored surface films formed from reactions of propanal in sulfuric acid at upper troposphere/lower stratosphere aerosol acidities.

    Science.gov (United States)

    Van Wyngarden, A L; Pérez-Montaño, S; Bui, J V H; Li, E S W; Nelson, T E; Ha, K T; Leong, L; Iraci, L T

    Particles in the upper troposphere and lower stratosphere (UT/LS) consist mostly of concentrated sulfuric acid (40-80 wt %) in water. However, airborne measurements have shown that these particles also contain a significant fraction of organic compounds of unknown chemical composition. Acid-catalyzed reactions of carbonyl species are believed to be responsible for significant transfer of gas phase organic species into tropospheric aerosols and are potentially more important at the high acidities characteristic of UT/LS particles. In this study, experiments combining sulfuric acid (H 2 SO 4 ) with propanal and with mixtures of propanal with glyoxal and/or methylglyoxal at acidities typical of UT/LS aerosols produced highly colored surface films (and solutions) that may have implications for aerosol properties. In order to identify the chemical processes responsible for the formation of the surface films, attenuated total reflectance-Fourier transform infrared (ATR-FTIR) and 1 H nuclear magnetic resonance (NMR) spectroscopies were used to analyze the chemical composition of the films. Films formed from propanal were a complex mixture of aldol condensation products, acetals and propanal itself. The major aldol condensation products were the dimer (2-methyl-2-pentenal) and 1,3,5-trimethylbenzene that was formed by cyclization of the linear aldol condensation trimer. Additionally, the strong visible absorption of the films indicates that higher-order aldol condensation products must also be present as minor species. The major acetal species were 2,4,6-triethyl-1,3,5-trioxane and longer-chain linear polyacetals which are likely to separate from the aqueous phase. Films formed on mixtures of propanal with glyoxal and/or methylglyoxal also showed evidence of products of cross-reactions. Since cross-reactions would be more likely than self-reactions under atmospheric conditions, similar reactions of aldehydes like propanal with common aerosol organic species like glyoxal

  9. Parameterization of the middle and upper tropospheric water vapor from ATOVS observations over a tropical climate region

    Science.gov (United States)

    Makama, Ezekiel Kaura; Lim, Hwee San; Abdullah, Khiruddin

    2018-01-01

    Precipitable water vapor (PWV) is a highly variable, but important greenhouse gas that regulates the radiation budget of the earth. Its variability in time and space makes it difficult to quantify. Knowledge of its vertical distribution, in particular, is crucial for many reasons. In this study, empirical relationships between isobaric layers of PWV over Peninsular Malaysia are examined. Analysis of variance (ANOVA) technique on Advanced Television and Infrared Observation Satellite Operational Vertical Sounder (ATOVS) observations, from 2005 to 2011, has been used to propose a relationship of the form, W=α(WL)β for the middle (MW) and upper (UW) layers PWV. W is either MW or UW with α and β as regression coefficients, which are functions of latitude. Coefficients of determination (R2) and root mean square error (RMSE) of respective values between 0.75-0.86 and 1.65-2.38 mm, across the zones, were obtained for both the MW and UW predictions, with a mean bias (MB) below ±1 mm.The predicted and observed PWV presented a better agreement northerly. Initial predictability test for each model was done on two independent data sets: ATOVS (2012-2015), and radiosonde (2010-2011) at Penang, Kuantan and Sepang stations, with very good outcomes. The results of the tests revealed remarkable performances, when compared with two previously reported models. The inclusion of variable regression coefficients, and the utilization of satellite-derived data, which provide soundings of data-void regions between radiosonde networks, proved to have optimized the results.

  10. A new cavity ring-down instrument for airborne monitoring of N2O5, NO3, NO2 and O3 in the upper troposphere lower stratosphere

    Science.gov (United States)

    Ruth, Albert A.; Brown, Steven S.; Dinesan, Hemanth; Dubé, William P.; Goulette, Marc; Hübler, Gerhard; Orphal, Johannes; Zahn, Andreas

    2016-04-01

    The chemistry of NO3 and N2O5 is important to the regulation of both tropospheric and stratospheric ozone. In situ detection of NO3 and N2O5 in the upper troposphere lower stratosphere (UTLS) represents a new scientific direction as the only previous measurements of these species in this region of the atmosphere has been via remote sensing techniques. Because both the sources and the sinks for NO3 and N2O5 are potentially stratified spatially, their mixing ratios, and their influence on nitrogen oxide and ozone transport and loss at night can show large variability as a function of altitude. Aircraft-based measurements of heterogeneous N2O5 uptake in the lower troposphere have uncovered a surprising degree of variability in the uptake coefficient [1], but there are no corresponding high altitude measurements.The UTLS is routinely sampled by the IAGOS-CARIBIC program (Civil Aircraft for the Regular Investigation of the atmosphere Based on an Instrument Container, www.caribic-atmospheric.com), a European infrastructural program with the aim of studying the chemistry and transport across this part of the atmosphere. An airfreight container with 15 different automated instruments from 8 European research partners is utilized on board a commercial Lufthansa airbus 340-600 to monitor ~ 100 atmospheric species (trace gases and aerosol parameters) in the UTLS. The instrumentation in the CARIBIC container is now to be supplemented by a new cavity ring-down device for monitoring nitrogen oxides, jointly developed by researchers from Cork (Ireland), Boulder (USA) and Karlsruhe (Germany). The compact and light-weight instrument is designed to monitor not only NO3 and N2O5, but also NO2 and O3. The detection is based on 4 high-finesse optical cavities (cavity length ~ 44 cm). Two cavities are operated at 662 nm (maximum absorption of NO3), the other two at 405 nm (maximum absorption of NO2). The inlet to one of the (662)-cavities is heated in order to thermally decompose N2O5

  11. Atmospheric statistical dynamic models. Climate experiments: albedo experiments with a zonal atmospheric model

    International Nuclear Information System (INIS)

    Potter, G.L.; Ellsaesser, H.W.; MacCracken, M.C.; Luther, F.M.

    1978-06-01

    The zonal model experiments with modified surface boundary conditions suggest an initial chain of feedback processes that is largest at the site of the perturbation: deforestation and/or desertification → increased surface albedo → reduced surface absorption of solar radiation → surface cooling and reduced evaporation → reduced convective activity → reduced precipitation and latent heat release → cooling of upper troposphere and increased tropospheric lapse rates → general global cooling and reduced precipitation. As indicated above, although the two experiments give similar overall global results, the location of the perturbation plays an important role in determining the response of the global circulation. These two-dimensional model results are also consistent with three-dimensional model experiments. These results have tempted us to consider the possibility that self-induced growth of the subtropical deserts could serve as a possible mechanism to cause the initial global cooling that then initiates a glacial advance thus activating the positive feedback loop involving ice-albedo feedback (also self-perpetuating). Reversal of the cycle sets in when the advancing ice cover forces the wave-cyclone tracks far enough equatorward to quench (revegetate) the subtropical deserts

  12. Overview of zonal flow physics

    International Nuclear Information System (INIS)

    Diamond, P.H.; Itoh, K.; Itoh, S.-I.; Hahm, T.S.

    2005-01-01

    Zonal flows, by which we mean azimuthally symmetric band-like shear flows, are ubiquitous phenomena in nature and the laboratory. It is now widely recognized that zonal flows are a key constituent in virtually all cases and regimes of drift wave turbulence, indeed, so much so that this classic problem is now frequently referred to as 'drift wave-zonal flow turbulence'. In this theory overview, we present new viewpoints and unifying concepts which facilitate understanding of zonal flow physics, via theory, computation and their confrontation with the results of laboratory experiment. Special emphasis is placed on identifying avenues for further progress. (author)

  13. Trace gas composition in the free and upper troposphere over Asia: Examining the influence of long-range transport and convection of local pollution

    Science.gov (United States)

    Baker, A. K.; Traud, S.; Brenninkmeijer, C. A.; Hoor, P. M.; Neumaier, M.; Oram, D.; Rauthe-Schöch, A.; Schloegl, S.; Sprung, D.; Slemr, F.; van Velthoven, P.; Wernli, H.; Zahn, A.; Ziereis, H.

    2013-12-01

    Between May 2005 and March 2008 the CARIBIC observatory (Civil Aircraft for the Regular Investigation of the atmosphere Based on an Instrument Container) was deployed to make atmospheric observations during 21 round-trip flights between Frankfurt, Germany and Manila, the Philippines with a stopover in Guangzhou, China. This nearly 3 year flight series provides us with information about atmospheric composition in the free and upper troposphere over Asia during all seasons and was used to investigate seasonal and regional differences in trace gas distributions and the relative influences of long range transport and convected local air masses on composition. The flight route was separated into three different regions having unique characteristics in transport and composition; these were Western Asia (5°E to 70°E), Central Asia (70°E to 100°E) and East Asia (100°E to 125°E). The region over Western Asia was heavily influenced by long range transport of air masses from North America and had elevated levels of NOy and acetone, while the region over East Asia was mostly influenced by convected local (South East Asian) pollution, particularly from biomass/biofuel burning as indicated by high levels of acetonitrile and carbon monoxide. Air masses over Central Asia were found to be influenced by both recently convected air masses from the Indian subcontinent and mid-range transport from Eastern Europe and the Middle East. Elevated levels of propane and other non-methane hydrocarbons, both with and without concommitant elevations in other trace gases (i.e. carbon monoxide, acetonitrile) were a persisent feature of this region in all seasons except summer, and were particularly prominent in fall. Influences on composition over Central Asia were investigated more thoroughly in a case study from a series of flights in October 2006, and elevated levels of pollutants were found to be the result of convective transport of both biomass/biofuel burning and urban emissions from

  14. Airborne differential absorption lidar for water vapour measurements in the upper troposphere and lower stratosphere in the spectral region around 940 nm

    Energy Technology Data Exchange (ETDEWEB)

    Poberaj, G.

    2000-07-01

    Two all-solid-state laser systems were developed and studied in detail to optimise their performance for an airborne water vapour differential absorption lidar (DIAL). Their special features are high average output powers and excellent spectral properties in the 940-nm spectral region relevant for monitoring very low water vapour contents in the upper troposphere and lower stratosphere. One system is an injection-seeded pulsed Ti:sapphire ring laser with a spectral bandwidth of 105 MHz and an average power of 1.1 W. The other system is an injection-seeded optical parametric oscillator (OPO) in a ring configuration. Using KTP as nonlinear crystal, a signal output with a spectral bandwidth of 140 MHz and an average power of 1.2 W was achieved. Both systems, the Ti:sapphire ring laser and the KTP OPO, possess spectral purity values higher than 99%. The pump source for these systems is a frequency doubled diode-pumped Nd:YAG laser operating at a repetition rate of 100 Hz. The KTP OPO system has been used as a transmitter in a new airborne water vapour DIAL instrument. For the first time, measurements of two-dimensional water vapour distributions with a high vertical (500 m) and horizontal (20 km) resolution across several potential vorticity streamers were performed. Very low water vapour mixing ratios (10-50 ppmv) and strong gradients were observed in the tropopause region. The sensitivity of the DIAL instrument in the centre of a stratospheric intrusion ranges from 3% in the near field to 12% in the far field (4 km). The first comparison experiments with in situ measuring instruments show a good agreement. Considerable differences are found between DIAL measurements and data obtained from the ECMWF operational analyses and a mesoscale numerical model. (orig.)

  15. Methyl chloride in the upper troposphere observed by the CARIBIC passenger aircraft observatory: Large-scale distributions and Asian summer monsoon outflow

    Science.gov (United States)

    Umezawa, T.; Baker, A. K.; Oram, D.; Sauvage, C.; O'Sullivan, D.; Rauthe-Schöch, A.; Montzka, S. A.; Zahn, A.; Brenninkmeijer, C. A. M.

    2014-05-01

    We present spatial and temporal variations of methyl chloride (CH3Cl) in the upper troposphere (UT) observed mainly by the Civil Aircraft for Regular Investigation of the atmosphere Based on an Instrument Container (CARIBIC) passenger aircraft for the years 2005-2011. The CH3Cl mixing ratio in the UT over Europe was higher than that observed at a European surface baseline station throughout the year, indicative of a persistent positive vertical gradient at Northern Hemisphere midlatitudes. A series of flights over Africa and South Asia show that CH3Cl mixing ratios increase toward tropical latitudes, and the observed UT CH3Cl level over these two regions and the Atlantic was higher than that measured at remote surface sites. Strong emissions of CH3Cl in the tropics combined with meridional air transport through the UT may explain such vertical and latitudinal gradients. Comparisons with carbon monoxide (CO) data indicate that noncombustion sources in the tropics dominantly contribute to forming the latitudinal gradient of CH3Cl in the UT. We also observed elevated mixing ratios of CH3Cl and CO in air influenced by biomass burning in South America and Africa, and the enhancement ratios derived for CH3Cl to CO in those regions agree with previous observations. In contrast, correlations indicate a high CH3Cl to CO ratio of 2.9 ± 0.5 ppt ppb-1 in the Asian summer monsoon anticyclone and domestic biofuel emissions in South Asia are inferred to be responsible. We estimated the CH3Cl emission in South Asia to be 134 ± 23 Gg Cl yr-1, which is higher than a previous estimate due to the higher CH3Cl to CO ratio observed in this study.

  16. Measurement of low-ppm mixing ratios of water vapor in the upper troposphere and lower stratosphere using chemical ionization mass spectrometry

    Directory of Open Access Journals (Sweden)

    T. D. Thornberry

    2013-06-01

    Full Text Available A chemical ionization mass spectrometer (CIMS instrument has been developed for the fast, precise, and accurate measurement of water vapor (H2O at low mixing ratios in the upper troposphere and lower stratosphere (UT/LS. A low-pressure flow of sample air passes through an ionization volume containing an α-particle radiation source, resulting in a cascade of ion-molecule reactions that produce hydronium ions (H3O+ from ambient H2O. The production of H3O+ ions from ambient H2O depends on pressure and flow through the ion source, which were tightly controlled in order to maintain the measurement sensitivity independent of changes in the airborne sampling environment. The instrument was calibrated every 45 min in flight by introducing a series of H2O mixing ratios between 0.5 and 153 parts per million (ppm, 10−6 mol mol−1 generated by Pt-catalyzed oxidation of H2 standards while overflowing the inlet with dry synthetic air. The CIMS H2O instrument was deployed in an unpressurized payload area aboard the NASA WB-57F high-altitude research aircraft during the Mid-latitude Airborne Cirrus Properties Experiment (MACPEX mission in March and April 2011. The instrument performed successfully during seven flights, measuring H2O mixing ratios below 5 ppm in the lower stratosphere at altitudes up to 17.7 km, and as low as 3.5 ppm near the tropopause. Data were acquired at 10 Hz and reported as 1 s averages. In-flight calibrations demonstrated a typical sensitivity of 2000 Hz ppm−1 at 3 ppm with a signal to noise ratio (2 σ, 1 s greater than 32. The total measurement uncertainty was 9 to 11%, derived from the uncertainty in the in situ calibrations.

  17. Transport pathways of CO in the African upper troposphere during the monsoon season: a study based upon the assimilation of spaceborne observations

    Directory of Open Access Journals (Sweden)

    B. Barret

    2008-06-01

    Full Text Available The transport pathways of carbon monoxide (CO in the African Upper Troposphere (UT during the West African Monsoon (WAM is investigated through the assimilation of CO observations by the Aura Microwave Limb Sounder (MLS in the MOCAGE Chemistry Transport Model (CTM. The assimilation setup, based on a 3-D First Guess at Assimilation Time (3-D-FGAT variational method is described. Comparisons between the assimilated CO fields and in situ airborne observations from the MOZAIC program between Europe and both Southern Africa and Southeast Asia show an overall good agreement around the lowermost pressure level sampled by MLS (~215 hPa. The 4-D assimilated fields averaged over the month of July 2006 have been used to determine the main dynamical processes responsible for the transport of CO in the African UT. The studied period corresponds to the second AMMA (African Monsoon Multidisciplinary Analyses aircraft campaign. At 220 hPa, the CO distribution is characterized by a latitudinal maximum around 5° N mostly driven by convective uplift of air masses impacted by biomass burning from Southern Africa, uplifted within the WAM region and vented predominantly southward by the upper branch of the winter hemisphere Hadley cell. Above 150 hPa, the African CO distribution is characterized by a broad maximum over northern Africa. This maximum is mostly controlled by the large scale UT circulation driven by the Asian Summer Monsoon (ASM and characterized by the Asian Monsoon Anticyclone (AMA centered at 30° N and the Tropical Easterly Jet (TEJ on the southern flank of the anticyclone. Asian pollution uplifted to the UT over large region of Southeast Asia is trapped within the AMA and transported by the anticyclonic circulation over Northeast Africa. South of the AMA, the TEJ is responsible for the tranport of CO-enriched air masses from India and Southeast Asia over Africa. Using the high time resolution provided by the 4-D assimilated fields, we give evidence

  18. Effects of 1997-1998 El Nino on Tropospheric Ozone and Water Vapor

    Science.gov (United States)

    Chandra, S.; Ziemke, J. R.; Min, W.; Read, W. G.

    1998-01-01

    This paper analyzes the impact of the 1997-1998 El Nino on tropospheric column ozone and tropospheric water vapor derived respectively from the Total Ozone Mapping Spectrometer (TOMS) on Earth Probe and the Microwave Limb Scanning instrument on the Upper Atmosphere Research Satellite. The 1997-1998 El Nino, characterized by an anomalous increase in sea-surface temperature (SST) across the eastern and central tropical Pacific Ocean, is one of the strongest El Nino Southern Oscillation (ENSO) events of the century, comparable in magnitude to the 1982-1983 episode. The major impact of the SST change has been the shift in the convection pattern from the western to the eastern Pacific affecting the response of rain-producing cumulonimbus. As a result, there has been a significant increase in rainfall over the eastern Pacific and a decrease over the western Pacific and Indonesia. The dryness in the Indonesian region has contributed to large-scale burning by uncontrolled wildfires in the tropical rainforests of Sumatra and Borneo. Our study shows that tropospheric column ozone decreased by 4-8 Dobson units (DU) in the eastern Pacific and increased by about 10-20 DU in the western Pacific largely as a result of the eastward shift of the tropical convective activity as inferred from National Oceanic and Atmospheric Administration (NOAA) outgoing longwave radiation (OLR) data. The effect of this shift is also evident in the upper tropospheric water vapor mixing ratio which varies inversely as ozone (O3). These conclusions are qualitatively consistent with the changes in atmospheric circulation derived from zonal and vertical wind data obtained from the Goddard Earth Observing System data assimilation analyses. The changes in tropospheric column O3 during the course of the 1997-1998 El Nino appear to be caused by a combination of large-scale circulation processes associated with the shift in the tropical convection pattern and surface/boundary layer processes associated with

  19. Impact of West African Monsoon convective transport and lightning NOx production upon the upper tropospheric composition: a multi-model study

    Directory of Open Access Journals (Sweden)

    H. Schlager

    2010-06-01

    Full Text Available Within the African Monsoon Multidisciplinary Analysis (AMMA, we investigate the impact of nitrogen oxides produced by lightning (LiNOx and convective transport during the West African Monsoon (WAM upon the composition of the upper troposphere (UT in the tropics. For this purpose, we have performed simulations with 4 state-of-the-art chemistry transport models involved within AMMA, namely MOCAGE, TM4, LMDz-INCA and p-TOMCAT. The model intercomparison is complemented with an evaluation of the simulations based on both spaceborne and airborne observations. The baseline simulations show important differences between the UT CO and O3 distributions simulated by each of the 4 models when compared to measurements from the MOZAIC program and fom the Aura/MLS spaceborne sensor. We show that such model discrepancies can be explained by differences in the convective transport parameterizations and, more particularly, the altitude reached by convective updrafts (ranging between ~200–125 hPa. Concerning UT O3, the models exhibit a good agreement with the main observed features. Nevertheless the majority of models simulate low O3 concentrations compared to both MOZAIC and Aura/MLS observations south of the equator, and rather high concentrations in the Northern Hemisphere. Sensitivity studies are performed to quantify the effect of deep convective transport and the influence of LiNOx production on the UT composition. These clearly indicate that the CO maxima and the elevated O3 concentrations south of the equator are due to convective uplift of air masses impacted by Southern African biomass burning, in agreement with previous studies. Moreover, during the WAM, LiNOx from Africa are responsible for the highest UT O3 enhancements (10–20 ppbv over the tropical Atlantic between 10° S–20° N. Differences between models are primarily due to the performance of the parameterizations used to simulate lightning activity which are evaluated using spaceborne

  20. The Role of Convection in Redistributing Formaldehyde to the Upper Troposphere Over North America and the North Atlantic during the Summer 2004 INTEX Campaign

    Science.gov (United States)

    Fried, Alan; Olson, Jennifer R.; Walega, Jim; Crawford, Jim H.; Chen, Gao; Weibring, Petter; Richter, Dirk; Roller, Chad; Tittel, Frank; Porter, Michael; hide

    2007-01-01

    Measurements of CH2O from a tunable diode laser absorption spectrometer (TDLAS) were acquired onboard the NASA DC-8 during the summer 2004 INTEX-NA (Intercontinental Chemical Transport Experiment - North America) campaign to test our understanding of convection and production mechanisms in the upper troposphere (UT, 6-12-km) over continental North America and the North Atlantic Ocean. Point-by-point comparisons with box model calculations, when MHP (CH3OOH) measurements were available for model constraint, resulted in a median CH2O measurement/model ratio of 0.91 in the UT. Multiple tracers were used to arrive at a set of UT CH2O background and perturbed air mass periods, and 46% of the TDLAS measurements fell within the latter category. At least 66% to 73% of these elevated UT observations were caused by enhanced production from CH2O precursors rather than direct transport of CH2O from the boundary layer. This distinction is important, since the effects from the former can last for over a week or more compared to one day or less in the case of convective transport of CH2O itself. In general, production of CH2O from CH4 was found to be the dominant source term, even in perturbed air masses. This was followed by production from MHP, methanol, PAN type compounds, and ketones, in descending order of their contribution. In the presence of elevated NO from lightning and potentially from the stratosphere, there was a definite trend in the CH2O discrepancy, which for the highest NO mixing ratios produced a median CH2O measurement/model ratio of 3.9 in the 10-12-km range. Discrepancies in CH2O and HO2 in the UT with NO were highly correlated and this provided further information as to the possible mechanism(s) responsible. These discrepancies with NO are consistent with additional production sources of both gases involving CH3O2 + NO reactions, most likely caused by unmeasured hydrocarbons.

  1. Model study of the impacts of emissions, chemical and dynamical processes on the CO variability in the tropical upper troposphere and lower stratosphere

    Directory of Open Access Journals (Sweden)

    Chunxiao Wang

    2015-07-01

    Full Text Available The Whole Atmosphere Community Climate Model (WACCM is used to investigate the relative importance of CO emissions, chemical and dynamical processes on temporal variations of CO in the tropical upper troposphere (UT and the lower stratosphere (LS. The semi-annual oscillation (SAO in the tropical UT and the annual oscillation (AO in the tropical LS detected in the MLS CO observations can be well captured by the model. The model simulations reveal that the CO surface emissions explain most of the SAO signals in the tropical UT, with the remainder being attributed to dynamical and chemical processes. The CO AO in the LS primarily results from combined effects of dynamical and chemical processes while the dynamical and chemical processes make opposite contributions to the CO AO signals, consistent with the previous findings. Our analysis further reveals that CO surface emissions tend to weaken the amplitude of the CO annual cycle in the tropical LS, while the annual variations in the meridional component of the Brewer–Dobson (BD circulation can amplify the annual variations of CO above 30 hPa. The model simulations also indicate that the CO annual cycle in the LS has a mixed behaviour with the annual variations of tropical upwelling reflected in CO between ~70 and ~50 hPa and a standard tape-recorder signal above 50 hPa. Moreover, the AO signals of CO exist up to 10 hPa when the chemical processes are switched off. The temporal and spatial variations of CO in the UT and near the tropopause are mainly driven by the upward transport of CO by tropical deep convection and the Asian summer monsoon circulation. In the early stage of the South Asian summer monsoon over the Bay of Bengal and the South China in the late spring and early summer, the transport of the CO surface emissions over Southeast Asia by the South Asian summer monsoon leads to an increase in the tropical CO, but the horizontal transport from the extratropics into the tropics (termed in

  2. On the wave forcing of the semi-annual zonal wind oscillation

    Science.gov (United States)

    Nagpal, O. P.; Raghavarao, R.

    1991-01-01

    Observational evidence of rather large period waves (23-60 d) in the troposphere/stratosphere, particularly during the winter months, is presented. Wind data collected on a regular basis employing high-altitude balloons and meteorological rockets over the past few years are used. Maximum entropy methods applied to the time series of zonal wind data indicate the presence of 23-60-waves more prominently than shorter-period waves. The waves have substantial amplitudes in the stratosphere and lower mesosphere, often larger than those noted in the troposphere. The mean zonal wind in the troposphere (5-15 km altitude) during December, January, and February exhibits the presence of strong westerlies at latitudes between 8 and 21 deg N.

  3. In situ measurements of tropical cloud properties in the West African Monsoon: upper tropospheric ice clouds, Mesoscale Convective System outflow, and subvisual cirrus

    Directory of Open Access Journals (Sweden)

    W. Frey

    2011-06-01

    Full Text Available In situ measurements of ice crystal size distributions in tropical upper troposphere/lower stratosphere (UT/LS clouds were performed during the SCOUT-AMMA campaign over West Africa in August 2006. The cloud properties were measured with a Forward Scattering Spectrometer Probe (FSSP-100 and a Cloud Imaging Probe (CIP operated aboard the Russian high altitude research aircraft M-55 Geophysica with the mission base in Ouagadougou, Burkina Faso. A total of 117 ice particle size distributions were obtained from the measurements in the vicinity of Mesoscale Convective Systems (MCS. Two to four modal lognormal size distributions were fitted to the average size distributions for different potential temperature bins. The measurements showed proportionately more large ice particles compared to former measurements above maritime regions. With the help of trace gas measurements of NO, NOy, CO2, CO, and O3 and satellite images, clouds in young and aged MCS outflow were identified. These events were observed at altitudes of 11.0 km to 14.2 km corresponding to potential temperature levels of 346 K to 356 K. In a young outflow from a developing MCS ice crystal number concentrations of up to (8.3 ± 1.6 cm−3 and rimed ice particles with maximum dimensions exceeding 1.5 mm were found. A maximum ice water content of 0.05 g m−3 was observed and an effective radius of about 90 μm. In contrast the aged outflow events were more diluted and showed a maximum number concentration of 0.03 cm−3, an ice water content of 2.3 × 10−4 g m−3, an effective radius of about 18 μm, while the largest particles had a maximum dimension of 61 μm.

    Close to the tropopause subvisual cirrus were encountered four times at altitudes of 15 km to 16.4 km. The mean ice particle number concentration of these encounters was 0.01 cm−3 with maximum particle sizes of 130

  4. Hydrological controls on the tropospheric ozone greenhouse gas effect

    Directory of Open Access Journals (Sweden)

    Le Kuai

    2017-03-01

    Full Text Available The influence of the hydrological cycle in the greenhouse gas (GHG effect of tropospheric ozone (O3 is quantified in terms of the O3longwave radiative effect (LWRE, which is defined as the net reduction of top-of-atmosphere flux due to total tropospheric O3absorption. The O3LWRE derived from the infrared spectral measurements by Aura’s Tropospheric Emission Spectrometer (TES show that the spatiotemporal variation of LWRE is relevant to relative humidity, surface temperature, and tropospheric O3column. The zonally averaged subtropical LWRE is ~0.2 W m-2higher than the zonally averaged tropical LWRE, generally due to lower water vapor concentrations and less cloud coverage at the downward branch of the Hadley cell in the subtropics. The largest values of O3LWRE over the Middle East (>1 W/m2 are further due to large thermal contrasts and tropospheric ozone enhancements from atmospheric circulation and pollution. Conversely, the low O3LWRE over the Inter-Tropical Convergence Zone (on average 0.4 W m-2 is due to strong water vapor absorption and cloudiness, both of which reduce the tropospheric O3absorption in the longwave radiation. These results show that changes in the hydrological cycle due to climate change could affect the magnitude and distribution of ozone radiative forcing.

  5. Comparisons of the tropospheric specific humidity from GPS radio occultations with ERA-Interim, NASA MERRA, and AIRS data

    Science.gov (United States)

    Vergados, Panagiotis; Mannucci, Anthony J.; Ao, Chi O.; Verkhoglyadova, Olga; Iijima, Byron

    2018-03-01

    We construct a 9-year data record (2007-2015) of the tropospheric specific humidity using Global Positioning System radio occultation (GPS RO) observations from the Constellation Observing System for Meteorology, Ionosphere, and Climate (COSMIC) mission. This record covers the ±40° latitude belt and includes estimates of the zonally averaged monthly mean specific humidity from 700 up to 400 hPa. It includes three major climate zones: (a) the deep tropics (±15°), (b) the trade winds belts (±15-30°), and (c) the subtropics (±30-40°). We find that the RO observations agree very well with the European Centre for Medium-Range Weather Forecasts Re-Analysis Interim (ERA-Interim), the Modern-Era Retrospective Analysis for Research and Applications (MERRA), and the Atmospheric Infrared Sounder (AIRS) by capturing similar magnitudes and patterns of variability in the monthly zonal mean specific humidity and interannual anomaly over annual and interannual timescales. The JPL and UCAR specific humidity climatologies differ by less than 15 % (depending on location and pressure level), primarily due to differences in the retrieved refractivity. In the middle-to-upper troposphere, in all climate zones, JPL is the wettest of all data sets, AIRS is the driest of all data sets, and UCAR, ERA-Interim, and MERRA are in very good agreement, lying between the JPL and AIRS climatologies. In the lower-to-middle troposphere, we present a complex behavior of discrepancies, and we speculate that this might be due to convection and entrainment. Conclusively, the RO observations could potentially be used as a climate variable, but more thorough analysis is required to assess the structural uncertainty between centers and its origin.

  6. Sensitivity of Middle Atmospheric Temperature and Circulation in the UIUC Mesosphere-Stratosphere-Troposphere GCM to the Treatment of Subgrid-Scale Gravity-Wave Breaking

    Science.gov (United States)

    Yang, Fanglin; Schlesinger, Michael E.; Andranova, Natasha; Zubov, Vladimir A.; Rozanov, Eugene V.; Callis, Lin B.

    2003-01-01

    The sensitivity of the middle atmospheric temperature and circulation to the treatment of mean- flow forcing due to breaking gravity waves was investigated using the University of Illinois at Urbana-Champaign 40-layer Mesosphere-Stratosphere-Troposphere General Circulation Model (MST-GCM). Three GCM experiments were performed. The gravity-wave forcing was represented first by Rayleigh friction, and then by the Alexander and Dunkerton (AD) parameterization with weak and strong breaking effects of gravity waves. In all experiments, the Palmer et al. parameterization was included to treat the breaking of topographic gravity waves in the troposphere and lower stratosphere. Overall, the experiment with the strong breaking effect simulates best the middle atmospheric temperature and circulation. With Rayleigh friction and the weak breaking effect, a large warm bias of up to 60 C was found in the summer upper mesosphere and lower thermosphere. This warm bias was linked to the inability of the GCM to simulate the reversal of the zonal winds from easterly to westerly crossing the mesopause in the summer hemisphere. With the strong breaking effect, the GCM was able to simulate this reversal, and essentially eliminated the warm bias. This improvement was the result of a much stronger meridional transport circulation that possesses a strong vertical ascending branch in the summer upper mesosphere, and hence large adiabatic cooling. Budget analysis indicates that 'in the middle atmosphere the forces that act to maintain a steady zonal-mean zonal wind are primarily those associated with the meridional transport circulation and breaking gravity waves. Contributions from the interaction of the model-resolved eddies with the mean flow are small. To obtain a transport circulation in the mesosphere of the UIUC MST-GCM that is strong enough to produce the observed cold summer mesopause, gravity-wave forcing larger than 100 m/s/day in magnitude is required near the summer mesopause. In

  7. Effects of stratospheric aerosol surface processes on the LLNL two-dimensional zonally averaged model

    International Nuclear Information System (INIS)

    Connell, P.S.; Kinnison, D.E.; Wuebbles, D.J.; Burley, J.D.; Johnston, H.S.

    1992-01-01

    We have investigated the effects of incorporating representations of heterogeneous chemical processes associated with stratospheric sulfuric acid aerosol into the LLNL two-dimensional, zonally averaged, model of the troposphere and stratosphere. Using distributions of aerosol surface area and volume density derived from SAGE 11 satellite observations, we were primarily interested in changes in partitioning within the Cl- and N- families in the lower stratosphere, compared to a model including only gas phase photochemical reactions

  8. Tropospheric Aerosols

    Science.gov (United States)

    Buseck, P. R.; Schwartz, S. E.

    2003-12-01

    It is widely believed that "On a clear day you can see forever," as proclaimed in the 1965 Broadway musical of the same name. While an admittedly beautiful thought, we all know that this concept is only figurative. Aside from Earth's curvature and Rayleigh scattering by air molecules, aerosols - colloidal suspensions of solid or liquid particles in a gas - limit our vision. Even on the clearest day, there are billions of aerosol particles per cubic meter of air.Atmospheric aerosols are commonly referred to as smoke, dust, haze, and smog, terms that are loosely reflective of their origin and composition. Aerosol particles have arisen naturally for eons from sea spray, volcanic emissions, wind entrainment of mineral dust, wildfires, and gas-to-particle conversion of hydrocarbons from plants and dimethylsulfide from the oceans. However, over the industrial period, the natural background aerosol has been greatly augmented by anthropogenic contributions, i.e., those produced by human activities. One manifestation of this impact is reduced visibility (Figure 1). Thus, perhaps more than in other realms of geochemistry, when considering the composition of the troposphere one must consider the effects of these activities. The atmosphere has become a reservoir for vast quantities of anthropogenic emissions that exert important perturbations on it and on the planetary ecosystem in general. Consequently, much recent research focuses on the effects of human activities on the atmosphere and, through them, on the environment and Earth's climate. For these reasons consideration of the geochemistry of the atmosphere, and of atmospheric aerosols in particular, must include the effects of human activities. (201K)Figure 1. Impairment of visibility by aerosols. Photographs at Yosemite National Park, California, USA. (a) Low aerosol concentration (particulate matter of aerodynamic diameter less than 2.5 μm, PM2.5=0.3 μg m-3; particulate matter of aerodynamic diameter less than 10

  9. The behaviour of stratospheric and upper tropospheric ozone in high and mid latitudes; the role of ozone as a climate gas

    Energy Technology Data Exchange (ETDEWEB)

    Kyroe, M.; Rummukainen, M.; Kivi, R.; Turunen, T.; Karhu, J. [Finnish Meteorological Inst., Sodankylae (Finland); Taalas, P. [Finnish Meteorological Inst., Helsinki (Finland)

    1996-12-31

    During the past few years, the dual role that ozone plays in climate change has been becoming increasingly obvious. First, continuous thinning of the ozone layer has been evident, even in the high and middle latitudes in the northern hemisphere. Secondly, ozone is also a greenhouse gas, affecting radiative transfer. Increases in tropospheric ozone have a positive forcing, whereas decreases in stratospheric ozone cause a negative forcing. During the last six years, measurements on total ozone and the vertical distribution of ozone have been performed at the Sodankylae Observatory. At Jokioinen Observatory, measurements on total ozone have been performed since 1990 and measurements on the vertical distribution of ozone since 1993. The overall project has focused on extending the national data series on total ozone and the vertical distribution of ozone. At the same time, the study has contributed to the study of interannual variability of the ozone layer. This SILMU project took part in the large-scale research activities, in addition to performing national studies. The results confirm that there has been fast chemical ozone destruction in the high latitudes in the northern hemisphere. This was particularly evident in the last two winters, 1994/95 and 1995/96. The new data also allows better trend analyses to be made on ozone in high and mid latitudes

  10. The behaviour of stratospheric and upper tropospheric ozone in high and mid latitudes; the role of ozone as a climate gas

    Energy Technology Data Exchange (ETDEWEB)

    Kyroe, M; Rummukainen, M; Kivi, R; Turunen, T; Karhu, J [Finnish Meteorological Inst., Sodankylae (Finland); Taalas, P [Finnish Meteorological Inst., Helsinki (Finland)

    1997-12-31

    During the past few years, the dual role that ozone plays in climate change has been becoming increasingly obvious. First, continuous thinning of the ozone layer has been evident, even in the high and middle latitudes in the northern hemisphere. Secondly, ozone is also a greenhouse gas, affecting radiative transfer. Increases in tropospheric ozone have a positive forcing, whereas decreases in stratospheric ozone cause a negative forcing. During the last six years, measurements on total ozone and the vertical distribution of ozone have been performed at the Sodankylae Observatory. At Jokioinen Observatory, measurements on total ozone have been performed since 1990 and measurements on the vertical distribution of ozone since 1993. The overall project has focused on extending the national data series on total ozone and the vertical distribution of ozone. At the same time, the study has contributed to the study of interannual variability of the ozone layer. This SILMU project took part in the large-scale research activities, in addition to performing national studies. The results confirm that there has been fast chemical ozone destruction in the high latitudes in the northern hemisphere. This was particularly evident in the last two winters, 1994/95 and 1995/96. The new data also allows better trend analyses to be made on ozone in high and mid latitudes

  11. In-situ BrO measurements in the upper troposphere / lower stratosphere. Validation of the ENVISAT satellite measurements and photochemical model studies

    Energy Technology Data Exchange (ETDEWEB)

    Hrechanyy, S.

    2007-04-15

    and SCOUT-O3 in the 15-20 km altitude regime are at the low side of comparable DOAS measurements a CLaMS study of the evolution of Bry from the source gases has been carried out. For this purpose an ensemble of trajectories rising from the lower troposphere to the TTL within 6 to more than 90 days were initialized with observed mixing ratios in the boundary layer of all important organic bromine source gases and the free-up of Bry by chemical and photochemical reactions was simulated. Bromoform, CHBr3, was found to be the main source of inorganic bromine at the tropopause. The derived tropospheric lifetime of bromoform is 33 days. The modelled BrO mixing ratio at the tropopause (less than 2.5 pptv) is consistent with HALOX measurements which do not detect significant amounts of BrO there (<1-2 pptv). Therefore measurements of more than 4 pptv (as retrieved from SCIAMACHY) can only be explained trough processes not included in the model. (orig.)

  12. Mid-infrared spectroscopy of Uranus from the Spitzer Infrared Spectrometer: 1. Determination of the mean temperature structure of the upper troposphere and stratosphere

    Science.gov (United States)

    Orton, Glenn S.; Fletcher, Leigh N.; Moses, Julianne I.; Mainzer, Amy K.; Hines, Dean; Hammel, Heidi B.; Martin-Torres, F. Javier; Burgdorf, Martin; Merlet, Cecile; Line, Michael R.

    2014-11-01

    On 2007 December 16-17, spectra were acquired of the disk of Uranus by the Spitzer Infrared Spectrometer (IRS), ten days after the planet's equinox, when its equator was close to the sub-Earth point. This spectrum provides the highest-resolution broad-band spectrum ever obtained for Uranus from space, allowing a determination of the disk-averaged temperature and molecule composition to a greater degree of accuracy than ever before. The temperature profiles derived from the Voyager radio occultation experiment by Lindal et al. (Lindal, G.F., Lyons, J.R., Sweetnam, D.N., Eshleman, V.R., Hinson, D.P. [1987]. J. Geophys. Res. 92, 14987-15001) and revisions suggested by Sromovsky et al. (Sromovsky, L.A., Fry, P.A., Kim, J.H. [2011]. Icarus 215, 292-312) that match these data best are those that assume a high abundance of methane in the deep atmosphere. However, none of these model profiles provides a satisfactory fit over the full spectral range sampled. This result could be the result of spatial differences between global and low-latitudinal regions, changes in time, missing continuum opacity sources such as stratospheric hazes or unknown tropospheric constituents, or undiagnosed systematic problems with either the Voyager radio-occultation or the Spitzer IRS data sets. The spectrum is compatible with the stratospheric temperatures derived from the Voyager ultraviolet occultations measurements by Herbert et al. (Herbert, F. et al. [1987]. J. Geophys. Res. 92, 15093-15109), but it is incompatible with the hot stratospheric temperatures derived from the same data by Stevens et al. (Stevens, M.H., Strobel, D.F., Herbert, F.H. [1993]. Icarus 101, 45-63). Thermospheric temperatures determined from the analysis of the observed H2 quadrupole emission features are colder than those derived by Herbert et al. at pressures less than ∼1 μbar. Extrapolation of the nominal model spectrum to far-infrared through millimeter wavelengths shows that the spectrum arising solely from H2

  13. Distribution of tropical tropospheric water vapor

    Science.gov (United States)

    Sun, De-Zheng; Lindzen, Richard S.

    1993-01-01

    Utilizing a conceptual model for tropical convection and observational data for water vapor, the maintenance of the vertical distribution of the tropical tropospheric water vapor is discussed. While deep convection induces large-scale subsidence that constrains the turbulent downgradient mixing to within the convective boundary layer and effectively dries the troposphere through downward advection, it also pumps hydrometeors into the upper troposphere, whose subsequent evaporation appears to be the major source of moisture for the large-scale subsiding motion. The development of upper-level clouds and precipitation from these clouds may also act to dry the outflow, thus explaining the low relative humidity near the tropopause. A one-dimensional model is developed to simulate the mean vertical structure of water vapor in the tropical troposphere. It is also shown that the horizontal variation of water vapor in the tropical troposphere above the trade-wind boundary layer can be explained by the variation of a moisture source that is proportional to the amount of upper-level clouds. Implications for the nature of water vapor feedback in global warming are discussed.

  14. Effect of some climatic parameters on tropospheric and total ozone ...

    Indian Academy of Sciences (India)

    carbon, carbon monoxide, nitrogen dioxide, and sulphur dioxide) that are collected from India Meteo- rological Department .... and the upper troposphere is not only able to absorb ... lar traffic, thermal power plants, very busy ports, small and ...

  15. Structure and variances of equatorial zonal circulation in a multimodel ensemble

    Energy Technology Data Exchange (ETDEWEB)

    Yu, B. [Environment Canada, Climate Data and Analysis Section, Climate Research Division, Toronto, ON (Canada); Zwiers, F.W. [University of Victoria, Pacific Climate Impacts Consortium, Victoria, BC (Canada); Boer, G.J. [Environment Canada, Canadian Centre for Climate Modeling and Analysis, Climate Research Division, Victoria, BC (Canada); Ting, M.F. [Columbia University, Lamont-Doherty Earth Observatory, Palisades, NY (United States)

    2012-11-15

    The structure and variance of the equatorial zonal circulation, as characterized by the atmospheric mass flux in the equatorial zonal plane, is examined and inter-compared in simulations from 9 CMIP3 coupled climate models with multiple ensemble members and the NCEP-NCAR and ERA-40 reanalyses. The climate model simulations analyzed here include twentieth century (20C3M) and twenty-first century (SRES A1B) simulations. We evaluate the 20C3M modeled zonal circulations by comparing them with those in the reanalyses. We then examine the variability of the circulation, its changes with global warming, and the associated thermodynamic maintenance. The tropical zonal circulation involves three major components situated over the Pacific, Indian, and Atlantic oceans. The three cells are supported by the corresponding diabatic heating extending deeply throughout the troposphere, with heating centers apparent in the mid-troposphere. Seasonal features appear in the zonal circulation, including variations in its intensity and longitudinal migration. Most models, and hence the multi-model mean, represent the annual and seasonal features of the circulation and the associated heating reasonably well. The multi-model mean reproduces the observed climatology better than any individual model, as indicated by the spatial pattern correlation and mean square difference of the mass flux and the diabatic heating compared to the reanalysis based values. Projected changes in the zonal circulation under A1B forcing are dominated by mass flux changes over the Pacific and Indian oceans. An eastward shift of the Pacific Walker circulation is clearly evident with global warming, with anomalous rising motion apparent over the equatorial central Pacific and anomalous sinking motions in the west and east, which favors an overall strengthening of the Walker circulation. The zonal circulation weakens and shifts westwards over the Indian Ocean under external forcing, whereas it strengthens and shifts

  16. Dynamics of zonal flows in helical systems.

    Science.gov (United States)

    Sugama, H; Watanabe, T-H

    2005-03-25

    A theory for describing collisionless long-time behavior of zonal flows in helical systems is presented and its validity is verified by gyrokinetic-Vlasov simulation. It is shown that, under the influence of particles trapped in helical ripples, the response of zonal flows to a given source becomes weaker for lower radial wave numbers and deeper helical ripples while a high-level zonal-flow response, which is not affected by helical-ripple-trapped particles, can be maintained for a longer time by reducing their bounce-averaged radial drift velocity. This implies a possibility that helical configurations optimized for reducing neoclassical ripple transport can simultaneously enhance zonal flows which lower anomalous transport.

  17. UPPER TROPOSPHERIC ND STR TOSPHERIC OZONE OVER ...

    African Journals Online (AJOL)

    USER

    2015-03-26

    Mar 26, 2015 ... site free of anthropogenic emissions, can be representative ... et al., 2009).The reduction in production of ... over Nairobi are small, light instruments attached on a .... pollutants from the city of Nairobi. The ... transport. Figure 9 ...

  18. Zonal methods and computational fluid dynamics

    International Nuclear Information System (INIS)

    Atta, E.H.

    1985-01-01

    Recent advances in developing numerical algorithms for solving fluid flow problems, and the continuing improvement in the speed and storage of large scale computers have made it feasible to compute the flow field about complex and realistic configurations. Current solution methods involve the use of a hierarchy of mathematical models ranging from the linearized potential equation to the Navier Stokes equations. Because of the increasing complexity of both the geometries and flowfields encountered in practical fluid flow simulation, there is a growing emphasis in computational fluid dynamics on the use of zonal methods. A zonal method is one that subdivides the total flow region into interconnected smaller regions or zones. The flow solutions in these zones are then patched together to establish the global flow field solution. Zonal methods are primarily used either to limit the complexity of the governing flow equations to a localized region or to alleviate the grid generation problems about geometrically complex and multicomponent configurations. This paper surveys the application of zonal methods for solving the flow field about two and three-dimensional configurations. Various factors affecting their accuracy and ease of implementation are also discussed. From the presented review it is concluded that zonal methods promise to be very effective for computing complex flowfields and configurations. Currently there are increasing efforts to improve their efficiency, versatility, and accuracy

  19. Reactive Nitrogen, Ozone and Ozone Production in the Arctic Troposphere and the Impact of Stratosphere-Troposphere Exchange

    Science.gov (United States)

    Liang, Q.; Rodriquez, J. M.; Douglass, A. R.; Crawford, J. H.; Apel, E.; Bian, H.; Blake, D. R.; Brune, W.; Chin, M.; Colarco, P. R.; hide

    2011-01-01

    We analyze the aircraft observations obtained during the Arctic Research of the Composition of the Troposphere from Aircraft and Satellite (ARCTAS) mission together with the GEOS-5 CO simulation to examine O3 and NOy in the Arctic and sub-Arctic region and their source attribution. Using a number of marker tracers and their probability density distributions, we distinguish various air masses from the background troposphere and examine their contribution to NOx, O3, and O3 production in the Arctic troposphere. The background Arctic troposphere has mean O3 of approximately 60 ppbv and NOx of approximately 25 pptv throughout spring and summer with CO decreases from approximately 145 ppbv in spring to approximately 100 ppbv in summer. These observed CO, NOx and O3 mixing ratios are not notably different from the values measured during the 1988 ABLE-3A and the 2002 TOPSE field campaigns despite the significant changes in the past two decades in processes that could have changed the Arctic tropospheric composition. Air masses associated with stratosphere-troposphere exchange are present throughout the mid and upper troposphere during spring and summer. These air masses with mean O3 concentration of 140-160 ppbv are the most important direct sources of O3 in the Arctic troposphere. In addition, air of stratospheric origin is the only notable driver of net O3 formation in the Arctic due to its sustainable high NOx (75 pptv in spring and 110 pptv in summer) and NOy (approximately 800 pptv in spring and approximately 1100 pptv in summer) levels. The ARCTAS measurements present observational evidence suggesting significant conversion of nitrogen from HNO3 to NOx and then to PAN (a net formation of approximately 120 pptv PAN) in summer when air of stratospheric origin is mixed with tropospheric background during stratosphere-to-troposphere transport. These findings imply that an adequate representation of stratospheric O3 and NOy input are essential in accurately simulating O3

  20. Changes in the zonal mean flow, temperature, and planetary waves observed in the Northern Hemisphere mid-winter months during the last decades

    Science.gov (United States)

    Rakushina, E. V.; Ermakova, T. S.; Pogoreltsev, A. I.

    2018-06-01

    Four sets of data: the UK Met Office, Modern Era Retrospective-analysis for Research and Applications (MERRA), Japanese 55-year Reanalysis data (JRA-55), and ERA-Interim data (ERA) have been used to estimate the climatic variability of the zonal mean flow, temperature, and Stationary Planetary Waves (SPW1, SPW2) from the troposphere up to the lower mesosphere levels. The composites of the meteorological fields during mid-winter month have been averaged over the first (1995-2005) and second (2006-2016) 11 years intervals and have been compared mainly paying attention to interannual and intraseasonal variability. Results show that changes in the mean fields and SPW2 are weaker and statistical significance of these changes is lower in comparison with the changes observed in the intraseasonal variability of these characteristics. All data sets demonstrate a decrease of SPW1 amplitude at the higher-middle latitudes in the lower stratosphere and opposite effect in the upper stratosphere. However, there is an increase of the intraseasonal variability for all meteorological parameters and this rise is statistically significant. The results obtained show that UK Met Office data demonstrate stronger changes and increase of the intraseasonal variability in comparison with other data sets.

  1. Seasonal Variability of Saturn's Tropospheric Temperatures, Winds and Para-H2 from Cassini Far-IR Spectroscopy

    Science.gov (United States)

    Fletcher, Leigh N.; Irwin, P. G. J; Achterberg, R. K.; Orton, G. S.; Flasar, F. M.

    2015-01-01

    temperatures, para-H2 and winds. Quantitative differences between the Cassini and Voyager epochs suggest that the oscillation is not in phase with the seasonal cycle at these tropospheric depths (i.e., it should be described as quasi-periodic rather than 'semi annual'). Variability in the zonal wind field derived from latitudinal thermal gradients is small (less than 10 m/s per scale height near the tropopause) and mostly affects the broad retrograde jets, with the notable exception of large variability on the northern flank of the equatorial jet. The meridional potential vorticity (PV) gradient, and hence the 'staircase of PV' associated with spatial variations in the vigour of vertical mixing, has varied over the course of the mission but maintained its overall shape. PV gradients in latitude and altitude are used to estimate the atmospheric refractive index for the propagation of stationary planetary (Rossby) waves, predicting that such wave activity would be confined to regions of real refractivity (tropical regions plus bands at 35-45 in both hemispheres). The penetration depth of these regions into the upper troposphere is temporally variable (potentially associated with stratification changes), whereas the latitudinal structure is largely unchanged over time (associated with the zonal jet system).

  2. The global distribution of tropospheric NO{sub x} estimated by a 3-D chemical tracer model

    Energy Technology Data Exchange (ETDEWEB)

    Kraus, A B; Rohrer, F; Ehhalt, D H [Forschungszentrum Juelich GmbH (Germany). Inst. fuer Atmosphaerische Chemie

    1998-12-31

    The global distribution of NO{sub x} in the troposphere is calculated using a three-dimensional chemical tracer model with a simplified chemistry scheme for the tracers NO{sub x} {identical_to} NO + NO{sub 2} and HNO{sub 3}. At northern mid- and high latitudes, the calculated tropospheric NO{sub x} content is dominated by the surface source fossil fuel combustion. In the tropical free troposphere lightning discharges provide about 80% of the total NO{sub x} throughout the year. The zonally averaged fractional contribution of aircraft emissions strongly depends on season. The NO mixing ratios determined by the model show good overall agreement with corresponding zonal mean values observed during the STRATOZ III aircraft campaign in June. Over Canada, mixing ratios as high as 0.5-1.0 ppbv NO were measured during TROPOZ II, the origin of which is not yet understood. (author) 8 refs.

  3. The global distribution of tropospheric NO{sub x} estimated by a 3-D chemical tracer model

    Energy Technology Data Exchange (ETDEWEB)

    Kraus, A.B.; Rohrer, F.; Ehhalt, D.H. [Forschungszentrum Juelich GmbH (Germany). Inst. fuer Atmosphaerische Chemie

    1997-12-31

    The global distribution of NO{sub x} in the troposphere is calculated using a three-dimensional chemical tracer model with a simplified chemistry scheme for the tracers NO{sub x} {identical_to} NO + NO{sub 2} and HNO{sub 3}. At northern mid- and high latitudes, the calculated tropospheric NO{sub x} content is dominated by the surface source fossil fuel combustion. In the tropical free troposphere lightning discharges provide about 80% of the total NO{sub x} throughout the year. The zonally averaged fractional contribution of aircraft emissions strongly depends on season. The NO mixing ratios determined by the model show good overall agreement with corresponding zonal mean values observed during the STRATOZ III aircraft campaign in June. Over Canada, mixing ratios as high as 0.5-1.0 ppbv NO were measured during TROPOZ II, the origin of which is not yet understood. (author) 8 refs.

  4. Stratosphere-troposphere exchange in a summertime extratropical low: analysis

    Directory of Open Access Journals (Sweden)

    J. Brioude

    2006-01-01

    Full Text Available Ozone and carbon monoxide measurements sampled during two commercial flights in airstreams of a summertime midlatitude cyclone are analysed with a Lagrangian-based study (backward trajectories and a Reverse Domain Filling technique to gain a comprehensive understanding of transport effects on trace gas distributions. The study demonstrates that summertime cyclones can be associated with deep stratosphere-troposphere transport. A tropopause fold is sampled twice in its life cycle, once in the lower troposphere (O3≃100 ppbv; CO≃90 ppbv in the dry airstream of the cyclone, and again in the upper troposphere (O3≃200 ppbv; CO≃90 ppbv on the northern side of the large scale potential vorticity feature associated with baroclinic development. In agreement with the maritime development of the cyclone, the chemical composition of the anticyclonic portion of the warm conveyor belt outflow (O3≃40 ppbv; CO≃85 ppbv corresponds to the lowest mixing ratios of both ozone and carbon monoxide in the upper tropospheric airborne observations. The uncertain degree of confidence of the Lagrangian-based technique applied to a 100 km segment of upper level airborne observations with high ozone (200 ppbv and relatively low CO (80 ppbv observed northwest of the cyclone prevents identification of the ozone enrichment process of air parcels embedded in the cyclonic part of the upper level outflow of the warm conveyor belt. Different hypotheses of stratosphere-troposphere exchange are discussed.

  5. Building an Anisotropic Meniscus with Zonal Variations

    Science.gov (United States)

    Higashioka, Michael M.; Chen, Justin A.; Hu, Jerry C.

    2014-01-01

    Toward addressing the difficult problems of knee meniscus regeneration, a self-assembling process has been used to re-create the native morphology and matrix properties. A significant problem in such attempts is the recapitulation of the distinct zones of the meniscus, the inner, more cartilaginous and the outer, more fibrocartilaginous zones. In this study, an anisotropic and zonally variant meniscus was produced by self-assembly of the inner meniscus (100% chondrocytes) followed by cell seeding the outer meniscus (coculture of chondrocytes and meniscus cells). After 4 weeks in culture, the engineered, inner meniscus exhibited a 42% increase in both instantaneous and relaxation moduli and a 62% increase in GAG/DW, as compared to the outer meniscus. In contrast, the circumferential tensile modulus and collagen/DW of the outer zone was 101% and 129% higher, respectively, than the values measured for the inner zone. Furthermore, there was no difference in the radial tensile modulus between the control and zonal engineered menisci, suggesting that the inner and outer zones of the engineered zonal menisci successfully integrated. These data demonstrate that not only can biomechanical and biochemical properties be engineered to differ by the zone, but they can also recapitulate the anisotropic behavior of the knee meniscus. PMID:23931258

  6. The zonal-mean and regional tropospheric pressure responses to changes in ionospheric potential

    Science.gov (United States)

    Zhou, Limin; Tinsley, Brian; Wang, Lin; Burns, Gary

    2018-06-01

    Global reanalysis data reveal daily surface pressure responses to changes in the global ionospheric potential in both polar and sub-polar regions. We use 21 years of data to show that the pressure response to externally-induced ionospheric potential changes, that are due to the interplanetary magnetic field east-west (IMF By) component, are present in two separate decadal intervals, and follow the opposite ionospheric potential changes in the Arctic and Antarctic for a given By. We use the 4 years of available data to show that the pressure responses to changes in internally generated ionospheric potential, that are caused by low-latitude thunderstorms and highly electrified clouds, agree in sign and sensitivity with those externally generated. We have determined that the daily varying pressure responses are stronger in local winter and spring. The pressure responses at polar latitudes are predominantly over the Antarctic and Greenland ice caps, and those at sub-polar latitudes are of opposite sign, mainly over oceans. A lead-lag analysis confirms that the responses maximize within two days of the ionospheric potential input. Regions of surface pressure fluctuating by about 4 hPa in winter are found with ionospheric potential changes of about 40 kV. The consistent pressure response to the independent external and internal inputs strongly supports the reality of a cloud microphysical mechanism affected by the global electric circuit. A speculative mechanism involves the ionosphere-earth current density Jz, which produces space charge at cloud boundaries and electrically charged droplets and aerosol particles. Ultrafine aerosol particles, under the action of electro-anti-scavenging, are enabled to grow to condensation nuclei size, affecting cloud microphysics and cloud opacity and surface pressure on time scales of hours.

  7. The governing processes and timescales of stratosphere-to-troposphere transport and its contribution to ozone in the Arctic troposphere

    Science.gov (United States)

    Liang, Q.; Douglass, A. R.; Duncan, B. N.; Stolarski, R. S.; Witte, J. C.

    2009-05-01

    We used the seasonality of a combination of atmospheric trace gases and idealized tracers to examine stratosphere-to-troposphere transport and its influence on tropospheric composition in the Arctic. Maximum stratosphere-to-troposphere transport of CFCs and O3 occurs in April as driven by the Brewer-Dobson circulation. Stratosphere-troposphere exchange (STE) occurs predominantly between 40° N to 80° N with stratospheric influx in the mid-latitudes (30-70° N) accounting for 67-81% of the air of stratospheric origin in the Northern Hemisphere extratropical troposphere. Transport from the lower stratosphere to the lower troposphere (LT) takes three months on average, one month to cross the tropopause, the second month to travel from the upper troposphere (UT) to the middle troposphere (MT), and the third month to reach the LT. During downward transport, the seasonality of a trace gas can be greatly impacted by wet removal and chemistry. A comparison of idealized tracers with varying lifetimes suggests that when initialized with the same concentrations and seasonal cycles at the tropopause, trace gases that have shorter lifetimes display lower concentrations, smaller amplitudes, and earlier seasonal maxima during transport to the LT. STE contributes to O3 in the Arctic troposphere directly from the transport of O3 and indirectly from the transport of NOy. Direct transport of O3 from the stratosphere accounts for 78% of O3 in the Arctic UT with maximum contributions occurring from March to May. The stratospheric contribution decreases significantly in the MT/LT (20-25% of total O3) and shows a very weak March-April maximum. Our NOx budget analysis in the Arctic UT shows that during spring and summer, the stratospheric injection of NOy-rich air increases NOx concentrations above the 20 pptv threshold level, thereby shifting the Arctic UT from a regime of net photochemical ozone loss to one of net production with rates as high as +16 ppbv/month.

  8. Four-peak longitudinal distribution of the equatorial plasma bubbles observed in the topside ionosphere: Possible troposphere tide influence

    Science.gov (United States)

    Sidorova, L. N.; Filippov, S. V.

    2018-03-01

    In this paper we consider an idea of the troposphere tide influence on the character of the longitudinal variations in the distribution of the equatorial plasma bubbles (EPBs) observed in the topside ionosphere. For this purpose, the obtained EPB longitudinal patterns were compared with the thermosphere and ionosphere characteristics having the prominent "wave-like" longitudinal structures with wave number 4, which are uniquely associated with the influence of the troposphere DE3 tides. The characteristics of the equatorial mass density anomaly (EMA), equatorial ionization anomaly (EIA), zonal wind and pre-reversal E × B drift enhancement (PRE) were used for comparison. The equinox seasons during high solar activity were under consideration. It was obtained that the longitudinal patterns of the EMA and zonal wind show the surprising similarity with the EPB distributions (R ≅ 0.8, R ≅ 0.72). On the other hand, the resemblance with the ionosphere characteristics (EIA, PRE) is rather faint (R ≅ 0.37, R ≅ 0.12). It was shown that the thermosphere zonal winds are the most possible transfer mediator of the troposphere DE3 tide influence. The most successful moment for the transfer of the troposphere DE3 tide energy takes place in the beginning of the EPB production, namely, during the seed perturbation development.

  9. Zonal wind observations during a geomagnetic storm

    Science.gov (United States)

    Miller, N. J.; Spencer, N. W.

    1986-01-01

    In situ measurements taken by the Wind and Temperature Spectrometer (WATS) onboard the Dynamics Explorer 2 spacecraft during a geomagnetic storm display zonal wind velocities that are reduced in the corotational direction as the storm intensifies. The data were taken within the altitudes 275 to 475 km in the dusk local time sector equatorward of the auroral region. Characteristic variations in the value of the Dst index of horizontal geomagnetic field strength are used to monitor the storm evolution. The detected global rise in atmospheric gas temperature indicates the development of thermospheric heating. Concurrent with that heating, reductions in corotational wind velocities were measured equatorward of the auroral region. Just after the sudden commencement, while thermospheric heating is intense in both hemispheres, eastward wind velocities in the northern hemisphere show reductions ranging from 500 m/s over high latitudes to 30 m/s over the geomagnetic equator. After 10 hours storm time, while northern thermospheric heating is diminishing, wind velocity reductions, distinct from those initially observed, begin to develop over southern latitudes. In the latter case, velocity reductions range from 300 m/s over the highest southern latitudes to 150 m/s over the geomagnetic equator and extend into the Northern Hemisphere. The observations highlight the interhemispheric asymmetry in the development of storm effects detected as enhanced gas temperatures and reduced eastward wind velocities. Zonal wind reductions over high latitudes can be attributed to the storm induced equatorward spread of westward polar cap plasma convection and the resulting plasma-neutral collisions. However, those collisions are less significant over low latitudes; so zonal wind reductions over low latitudes must be attributed to an equatorward extension of a thermospheric circulation pattern disrupted by high latitude collisions between neutrals transported via eastward winds and ions

  10. Linear zonal atmospheric prediction for adaptive optics

    Science.gov (United States)

    McGuire, Patrick C.; Rhoadarmer, Troy A.; Coy, Hanna A.; Angel, J. Roger P.; Lloyd-Hart, Michael

    2000-07-01

    We compare linear zonal predictors of atmospheric turbulence for adaptive optics. Zonal prediction has the possible advantage of being able to interpret and utilize wind-velocity information from the wavefront sensor better than modal prediction. For simulated open-loop atmospheric data for a 2- meter 16-subaperture AO telescope with 5 millisecond prediction and a lookback of 4 slope-vectors, we find that Widrow-Hoff Delta-Rule training of linear nets and Back- Propagation training of non-linear multilayer neural networks is quite slow, getting stuck on plateaus or in local minima. Recursive Least Squares training of linear predictors is two orders of magnitude faster and it also converges to the solution with global minimum error. We have successfully implemented Amari's Adaptive Natural Gradient Learning (ANGL) technique for a linear zonal predictor, which premultiplies the Delta-Rule gradients with a matrix that orthogonalizes the parameter space and speeds up the training by two orders of magnitude, like the Recursive Least Squares predictor. This shows that the simple Widrow-Hoff Delta-Rule's slow convergence is not a fluke. In the case of bright guidestars, the ANGL, RLS, and standard matrix-inversion least-squares (MILS) algorithms all converge to the same global minimum linear total phase error (approximately 0.18 rad2), which is only approximately 5% higher than the spatial phase error (approximately 0.17 rad2), and is approximately 33% lower than the total 'naive' phase error without prediction (approximately 0.27 rad2). ANGL can, in principle, also be extended to make non-linear neural network training feasible for these large networks, with the potential to lower the predictor error below the linear predictor error. We will soon scale our linear work to the approximately 108-subaperture MMT AO system, both with simulations and real wavefront sensor data from prime focus.

  11. A consistent definition of the Arctic polar vortex breakup in both the lower and upper stratosphere

    Science.gov (United States)

    Choi, W.; Seo, J.

    2014-12-01

    Breakup of the polar vortex is a dominant feature of the seasonal transition from winter to summer in the stratosphere, which significantly affects stratospheric O3 concentration and tropospheric weather. Previously several criteria for the vortex breakup have been suggested based on the potential vorticity (PV) and wind speed, however, those mainly have focused on the lower stratospheric vortex of which spatiotemporal evolution and decay are more continuous than those of the upper stratospheric vortex. To find a consistent criterion for the vortex breakup in both the lower and upper stratosphere, the present study defined a polar vortex breakup day as when PV gradient at the polar vortex edge becomes lower than that at the subtropical edge on the area equivalent latitude based on PV. With applying the new definition to the UK Met Office reanalysis data, the breakup days of the Arctic polar vortices on 18 isentropic levels from 450 K to 1300 K were calculated for the period of 1993-2005. In comparison with CH4, N2O and O3 measured by the ILAS and POAM II/III satellite instruments, the breakup days are well consistent with changes in the distribution of such tracers as well as their zonal standard deviations associated with the vortex structure breaking and irreversible mixing. The vortex breakup in the upper stratosphere occurs more or less a month prior to that in the middle and lower stratosphere while the stratospheric final warming events occurs simultaneously in the upper and lower stratosphere.

  12. Numerical Simulation on Zonal Disintegration in Deep Surrounding Rock Mass

    OpenAIRE

    Xuguang Chen; Yuan Wang; Yu Mei; Xin Zhang

    2014-01-01

    Zonal disintegration have been discovered in many underground tunnels with the increasing of embedded depth. The formation mechanism of such phenomenon is difficult to explain under the framework of traditional rock mechanics, and the fractured shape and forming conditions are unclear. The numerical simulation was carried out to research the generating condition and forming process of zonal disintegration. Via comparing the results with the geomechanical model test, the zonal disintegration p...

  13. A Raman lidar at La Reunion (20.8° S, 55.5° E for monitoring water vapour and cirrus distributions in the subtropical upper troposphere: preliminary analyses and description of a future system

    Directory of Open Access Journals (Sweden)

    C. Hoareau

    2012-06-01

    Full Text Available A ground-based Rayleigh lidar has provided continuous observations of tropospheric water vapour profiles and cirrus cloud using a preliminary Raman channels setup on an existing Rayleigh lidar above La Reunion over the period 2002–2005. With this instrument, we performed a first measurement campaign of 350 independent water vapour profiles. A statistical study of the distribution of water vapour profiles is presented and some investigations concerning the calibration are discussed. Analysis regarding the cirrus clouds is presented and a classification has been performed showing 3 distinct classes. Based on these results, the characteristics and the design of a future lidar system, to be implemented at the new Reunion Island altitude observatory (2200 m for long-term monitoring, is presented and numerical simulations of system performance have been realised to compare both instruments.

  14. Tropospheric Ozone as a Short-lived Chemical Climate Forcer

    Science.gov (United States)

    Pickering, Kenneth E.

    2012-01-01

    Tropospheric ozone is the third most important greenhouse gas according to the most recent IPCC assessment. However, tropospheric ozone is highly variable in both space and time. Ozone that is located in the vicinity of the tropopause has the greatest effect on climate forcing. Nitrogen oxides (NOx) are the most important precursors for ozone In most of the troposphere. Therefore, pollution that is lofted upward in thunderstorm updrafts or NOx produced by lightning leads to efficient ozone production in the upper troposphere, where ozone is most important climatically. Global and regional model estimates of the impact of North American pollution and lightning on ozone radiative forcing will be presented. It will be shown that in the Northern Hemisphere summer, the lightning effect on ozone radiative forcing can dominate over that of pollution, and that the radiative forcing signal from North America extends well into Europe and North Africa. An algorithm for predicting lightning flash rates and estimating lightning NOx emissions is being incorporated into the NASA GEOS-5 Chemistry and Climate Model. Changes in flash rates and emissions over an ENSO cycle and in future climates will be assessed, along with the resulting changes in upper tropospheric ozone. Other research on the production of NOx per lightning flash and its distribution in the vertical based on cloud-resolving modeling and satellite observations will be presented. Distributions of NO2 and O3 over the Middle East from the OMI instrument on NASA's Aura satellite will also be shown.

  15. Currents, Geostrophic, Aviso, 0.25 degrees, Global, Zonal

    Data.gov (United States)

    National Oceanic and Atmospheric Administration, Department of Commerce — Aviso Zonal Geostrophic Current is inferred from Sea Surface Height Deviation, climatological dynamic height, and basic fluid mechanics.

  16. The residual zonal dynamics in a toroidally rotating tokamak

    International Nuclear Information System (INIS)

    Zhou Deng

    2015-01-01

    Zonal flows, initially driven by ion-temperature-gradient turbulence, may evolve due to the neoclassic polarization in a collisionless tokamak plasma. In this presentation, the form of the residual zonal flow is presented for tokamak plasmas rotating toroidally at arbitrary velocity. The gyro-kinetic equation is analytically solved to give the expression of residual zonal flows with arbitrary rotating velocity. The zonal flow level decreases as the rotating velocity increases. The numerical evaluation is in good agreement with the previous simulation result for high aspect ratio tokamaks. (author)

  17. Zonal flows in tokamaks with anisotropic pressure

    International Nuclear Information System (INIS)

    Ren, Haijun

    2014-01-01

    Zonal flows (ZFs) in a tokamak plasma with anisotropic pressure are investigated. The dynamics of perpendicular and parallel pressures are determined by the Chew-Goldberger-Low double equations and low-β condition is adopted, where β is the ratio of plasma pressure to the magnetic field pressure. The dispersion relation is analytically derived and illustrates two branches of ZFs. The low frequency zonal flow (LFZF) branch becomes unstable when χ, the ratio of the perpendicular pressure to the parallel one, is greater than a threshold value χ c , which is about 3.8. In the stable region, its frequency increases first and then decreases with increasing χ. For χ = 1, the frequency of LFZF agrees well with the experimental observation. For the instability, the growth rate of LFZF increases with χ. The geodesic acoustic mode branch is shown to be always stable with a frequency increasing with χ. The safety factor is shown to diminish the frequencies of both branches or the growth rate of LFZF

  18. Origins of Tropospheric Ozone Interannual Variation (IAV) over Reunion: A Model Investigation

    Science.gov (United States)

    Liu, Junhua; Rodriguez, Jose M.; Thompson, Anne M.; Logan, Jennifer A.; Douglass, Anne R.; Olsen, Mark A.; Steenrod, Stephen D.; Posny, Francoise

    2016-01-01

    Observations from long-term ozonesonde measurements show robust variations and trends in the evolution of ozone in the middle and upper troposphere over Reunion Island (21.1 degrees South Latitude, 55.5 degrees East Longitude) in June-August. Here we examine possible causes of the observed ozone variation at Reunion Island using hindcast simulations by the stratosphere-troposphere Global Modeling Initiative chemical transport model for 1992-2014, driven by assimilated Modern-Era Retrospective Analysis for Research and Applications (MERRA) meteorological fields. Reunion Island is at the edge of the subtropical jet, a region of strong stratospheric-tropospheric exchange. Our analysis implies that the large interannual variation (IAV) of upper tropospheric ozone over Reunion is driven by the large IAV of the stratospheric influence. The IAV of the large-scale, quasi-horizontal wind patterns also contributes to the IAV of ozone in the upper troposphere. Comparison to a simulation with constant emissions indicates that increasing emissions do not lead to the maximum trend in the middle and upper troposphere over Reunion during austral winter implied by the sonde data. The effects of increasing emission over southern Africa are limited tothe lower troposphere near the surface in August-September.

  19. Troposphere - ionosphere interaction during tropospheric MCC events

    International Nuclear Information System (INIS)

    Manzano, J.R.; Zossi Artigas, M.M. de; Filippi Manzano, A.N. de; Cosio Ragone, A.H. de

    1995-09-01

    The present paper describes the investigation of possible effects of the type of large meteorological events known as Mesoscale Convective Complexes (MCC) on the F-region of the ionosphere over Argentina. These warm-season weather systems of huge size are present in the United States (Maddox, 1980) and in South Americal (Velasco and Fritsch, 1987). Their extension can be as large as 1,300,000 Km 2 and they tend to move in different directions over the earth surface. It is expected that these meteorological events should leave its signature in the upper region of the atmosphere. 13 refs, 12 figs, 1 tab

  20. Tropospheric NO2 over China

    NARCIS (Netherlands)

    A, van der R.J.; Peters, D.H.M.U.; Kuenen, J.J.P.; Eskes, H.J.; Boersma, K.F.; Roozendael, Van M.; Smedt, de I.; Zhang, P.; Kelder, H.M.; Lacoste, H.; Ouwehand, L.

    2006-01-01

    The results are presented of a study to tropospheric NO2 over China, based on measurements from the satellite instruments GOME and SCIAMACHY. A data set of 10 year tropospheric NO2 has been processed from GOME and SCIAMACHY observations using a combined retrieval/assimilation approach. This approach

  1. Acute Zonal Cone Photoreceptor Outer Segment Loss.

    Science.gov (United States)

    Aleman, Tomas S; Sandhu, Harpal S; Serrano, Leona W; Traband, Anastasia; Lau, Marisa K; Adamus, Grazyna; Avery, Robert A

    2017-05-01

    The diagnostic path presented narrows down the cause of acute vision loss to the cone photoreceptor outer segment and will refocus the search for the cause of similar currently idiopathic conditions. To describe the structural and functional associations found in a patient with acute zonal occult photoreceptor loss. A case report of an adolescent boy with acute visual field loss despite a normal fundus examination performed at a university teaching hospital. Results of a complete ophthalmic examination, full-field flash electroretinography (ERG) and multifocal ERG, light-adapted achromatic and 2-color dark-adapted perimetry, and microperimetry. Imaging was performed with spectral-domain optical coherence tomography (SD-OCT), near-infrared (NIR) and short-wavelength (SW) fundus autofluorescence (FAF), and NIR reflectance (REF). The patient was evaluated within a week of the onset of a scotoma in the nasal field of his left eye. Visual acuity was 20/20 OU, and color vision was normal in both eyes. Results of the fundus examination and of SW-FAF and NIR-FAF imaging were normal in both eyes, whereas NIR-REF imaging showed a region of hyporeflectance temporal to the fovea that corresponded with a dense relative scotoma noted on light-adapted static perimetry in the left eye. Loss in the photoreceptor outer segment detected by SD-OCT co-localized with an area of dense cone dysfunction detected on light-adapted perimetry and multifocal ERG but with near-normal rod-mediated vision according to results of 2-color dark-adapted perimetry. Full-field flash ERG findings were normal in both eyes. The outer nuclear layer and inner retinal thicknesses were normal. Localized, isolated cone dysfunction may represent the earliest photoreceptor abnormality or a distinct entity within the acute zonal occult outer retinopathy complex. Acute zonal occult outer retinopathy should be considered in patients with acute vision loss and abnormalities on NIR-REF imaging, especially if

  2. Tropospheric Halogen Chemistry

    Science.gov (United States)

    von Glasow, R.; Crutzen, P. J.

    2003-12-01

    Halogens are very reactive chemicals that are known to play an important role in anthropogenic stratospheric ozone depletion chemistry, first recognized by Molina and Rowland (1974). However, they also affect the chemistry of the troposphere. They are of special interest because they are involved in many reaction cycles that can affect the oxidation power of the atmosphere indirectly by influencing the main oxidants O3 and its photolysis product OH and directly, e.g., by reactions of the Cl radical with hydrocarbons (e.g., CH4).Already by the middle of the nineteenth century, Marchand (1852) reported the presence of bromine and iodine in rain and other natural waters. He also mentions the benefits of iodine in drinking water through the prevention of goitres and cretinism. In a prophetic monograph "Air and Rain: The Beginnings of a Chemical Climatology," Smith (1872) describes measurements of chloride in rain water, which he states to originate partly from the oceans by a process that he compares with the bursting of "soap bubbles" which produces "small vehicles" that transfer small spray droplets of seawater to the air. From deviations of the sulfate-to-chloride ratio in coastal rain compared to seawater, Smith concluded that chemical processes occur once the particles are airborne.For almost a century thereafter, however, atmospheric halogens received little attention. One exception was the work by Cauer (1939), who reported that iodine pollution has been significant in Western and Central Europe due to the inefficient burning of seaweed, causing mean gas phase atmospheric concentrations as high as or greater than 0.5 μg m-3. In his classical textbook Air Chemistry and Radioactivity, Junge (1963) devoted less than three pages to halogen gas phase chemistry, discussing chlorine and iodine. As reviewed by Eriksson (1959a, b), the main atmospheric source of halogens is sea salt, derived from the bursting of bubbles of air which are produced by ocean waves and other

  3. Theory, simulation, and experimental studies of zonal flows

    International Nuclear Information System (INIS)

    Hahm, T. S.; Burrell, K.H.; Lin, Z.; Nazikian, R.; Synakowski, E.J.

    2000-01-01

    The authors report on current theoretical understanding of the characteristics of self-generated zonal flows as observed in nonlinear gyrokinetic simulations of toroidal ITG turbulence [Science 281, 1835 (1998)], and discuss various possibilities for experimental measurements of signature of zonal flows

  4. Thermospheric zonal mean winds and tides revealed by CHAMP

    NARCIS (Netherlands)

    Lieberman, R.S.; Akmaev, R.A.; Fuller-Rowell, T.J.; Doornbos, E.

    2013-01-01

    We present direct, global observations of longitudinally averaged CHAMP zonal winds gathered between 2003 and 2007. A diurnal variation dominates the global zonal wind. Westward flows are observed from the early morning through afternoon hours, while eastward flows peak in the evening. A semidiurnal

  5. Lidar investigations on the optical and dynamical properties of cirrus clouds in the upper troposphere and lower stratosphere regions at a tropical station, Gadanki, India (13.5°N, 79.2°E)

    Science.gov (United States)

    Krishnakumar, Vasudevannair; Satyanarayana, Malladi; Radhakrishnan, Soman R.; Dhaman, Reji K.; Jayeshlal, Glory Selvan; Motty, Gopinathan Nair S.; Pillai, Vellara P. Mahadevan; Raghunath, Karnam; Ratnam, Madineni Venkat; Rao, Duggirala Ramakrishna; Sudhakar, Pindlodi

    2014-01-01

    High altitude cirrus clouds are composed mainly of ice crystals with a variety of sizes and shapes. They have a large influence on Earth's energy balance and global climate. Recent studies indicate that the formation, dissipation, life time, optical, and micro-physical properties are influenced by the dynamical conditions of the surrounding atmosphere like background aerosol, turbulence, etc. In this work, an attempt has been made to quantify some of these characteristics by using lidar and mesosphere-stratosphere-troposphere (MST) radar. Mie lidar and 53 MHz MST radar measurements made over 41 nights during the period 2009 to 2010 from the tropical station, Gadanki, India (13.5°N, 79.2°E). The optical and microphysical properties along with the structure and dynamics of the cirrus are presented as observed under different atmospheric conditions. The study reveals the manifestation of different forms of cirrus with a preferred altitude of formation in the 13 to 14 km altitude. There are considerable differences in the properties obtained among 2009 and 2010 showing significant anomalous behavior in 2010. The clouds observed during 2010 show relatively high asymmetry and large multiple scattering effects. The anomalies found during 2010 may be attributed to the turbulence noticed in the surrounding atmosphere. The results show a clear correlation between the crystal morphology in the clouds and the dynamical conditions of the prevailing atmosphere during the observational period.

  6. Regulation of ETG turbulence by TEM driven zonal flows

    Science.gov (United States)

    Asahi, Yuuichi; Ishizawa, Akihiro; Watanabe, Tomohiko; Tsutsui, Hiroaki; Tsuji-Iio, Shunji

    2013-10-01

    Anomalous heat transport driven by electron temperature gradient (ETG) turbulence is investigated by means of gyrokinetic simulations. It is found that the ETG turbulence can be suppressed by zonal flows driven by trapped electron modes (TEMs). The TEMs appear in a statistically steady state of ETG turbulence and generate zonal flows, while its growth rate is much smaller than those of ETGs. The TEM-driven zonal flows with lower radial wave numbers are more strongly generated than those driven by ETG modes, because of the higher zonal flow response to a density source term. An ExB shearing rate of the TEM-driven zonal flows is strong enough to suppress the long-wavelength ETG modes which make the main contribution to the turbulent transport.

  7. Study on the regional and global rise in NO{sub x} and non-methane hydrocarbon concentrations in the upper troposphere and lower stratosphere as a consequence of airplane emissions. Final report; Untersuchungen zur regionalen und globalen Erhoehung der NO{sub x}- und Nichtmethankohlenwasserstoff-Konzentrationen in der oberen Troposphaere und der unteren Stratosphaere infolge Flugzeugemissionen. Abschlussbericht

    Energy Technology Data Exchange (ETDEWEB)

    Rohrer, F

    1996-01-05

    In this project a chemical mechanism was developed for the upper troposphere which permits examining the photochemical formation of ozone. Using this mechanism it was found that at medium latitudes (at 10 km altitude in June) hydroxyl radical concentration and the rate of photochemical ozone formation to which it is coupled depend on NO{sub x} concentrations in a strongly non-linear manner, peaking at 110 ppt NO{sub x} and 200 pp NO{sub x}, respectively. Regarding the assessment of the effects of air traffic it was thus shown that in attempting to forecast changes in ozone concentration one must not only take aviation-related changes in NO{sub x} concentrations into account but also the forecasted absolute concentrations of NO{sub x}. The measured data were interpreted by combining a simplified model of NO{sub x} reactions with an existing three-dimensional transport model and comparing the measured and the calculated vertical NO profiles. It can be said that the 3D chemical transport model supplies realistic tropospheric NO{sub x} ratios at least for medium latitudes (49 to 56 N) in the months of May, June, July, December, and January. At these latitudes the tropospheric NO{sub x} budget is mainly governed by anthropogenic emissions. (orig./KW) [Deutsch] In diesem Projekt wurde ein Chemiemechanismus fuer die obere Troposphaere entwickelt, der es erlaubt, die photochemische Ozonbildung zu untersuchen. Mit diesem Mechanismus konnte fuer mittlere noerdliche Breiten (fuer 10 km Hoehe, Juni) gezeigt werden, dass die Hydroxylradikalkonzentration und die damit gekoppelte photochemische Ozonbildungsrate in stark nichtlinearer Weise von der Stickoxidkonzentration abhaengen und bei etwa 110 ppt NO{sub x} (bezw. 200 ppt NO{sub x} fuer die Ozonbildungsrate) ein Maximum durchlaufen. Fuer die Beurteilung der Auswirkungen des Flugverkehrs konnte deswegen gezeigt werden, dass die Voraussagen ueber Ozonveraenderungen nicht nur von der Aenderung der Stickoxidkonzentration durch den

  8. An investigation of the processes controlling ozone in the upper stratosphere

    International Nuclear Information System (INIS)

    Patten, K.O. Jr.; Connell, P.S.; Kinnison, D.E.; Wuebbles, D.J.; Waters, J.; Froidevaux, L.; Slanger, T.G.

    1992-01-01

    Photolysis of vibrationally excited oxygen produced by ultraviolet photolysis of ozone in the upper stratosphere is incorporated into the Lawrence Livermore National Laboratory 2-D zonally averaged chemical-radiative-transport model of the troposphere and stratosphere. The importance of this potential contributor of odd oxygen to the concentration of ozone is evaluated based upon recent information on vibrational distributions of excited oxygen and upon preliminary studies of energy transfer from the excited oxygen. When the energy transfer rate constants of previous work are assumed, increases in model ozone concentrations of up to 40 percent in the upper stratosphere are found, and the ozone concentrations of the model agree with measurements, including data from the Upper Atmosphere Research Satellite. However, the increase is about 0.4 percent when the larger energy transfer rate constants suggested by more recent experimental work are applied in the model. This indicates the importance of obtaining detailed information on vibrationally excited oxygen properties, particularly the state-specific energy transfer rate constants, to evaluation of tills precess for stratospheric modeling

  9. Tropical Tropospheric Ozone from SHADOZ (Southern Hemisphere ADditional Ozonesondes) Network: A Project for Satellite Research, Process Studies, Education

    Science.gov (United States)

    Thompson, Anne M.; Witte, Jacquelyn C.; Oltmans, Samuel J.; Schmidlin, Francis J.; Coetzee, G. J. R.; Hoegger, Bruno; Kirchhoff, V. W. J. H.; Ogawa, Toshihiro; Kawakami, Shuji; Posny, Francoise

    2002-01-01

    The first climatological overview of total, stratospheric and tropospheric ozone in the southern hemisphere tropical and subtropics is based on ozone sounding data from 10 sites comprising the Southern Hemisphere Additional OZonesondes (SHADOZ) network. The period covered is 1998-2000. Observations were made over: Ascension Island; Nairobi, Kenya; Irene, South Africa; Reunion Island; Watukosek, Java; Fiji; Tahiti; American Samoa; San Cristobal, Galapagos; Natal, Brazil. Campaign data were collected on a trans-Atlantic oceanographic cruise and during SAFARI-2000 in Zambia. The ozone data, with simultaneous temperature profiles to approx. 7 hPa and relative humidity to approx. 200 hPa, reside at: . SHADOZ ozone time-series and profiles give a perspective on tropical total, stratospheric and tropospheric ozone. Prominent features are highly variable tropospheric ozone and a zonal wave-one pattern in total (and tropospheric) column ozone. Total, stratospheric and tropospheric column ozone amounts peak between August and November and are lowest between March and May. Tropospheric ozone variability over the Indian and Pacific Ocean displays influences of the Indian Ocean Dipole and convective mixing. Pollution transport from Africa and South America is a seasonal feature. Tropospheric ozone seasonality over the Atlantic Basin shows effects of regional subsidence and recirculation as well as biomass burning. Dynamical and chemical influences appear to be of comparable magnitude though model studies are needed to quantify this.

  10. Thermodynamic constraint on the depth of the global tropospheric circulation.

    Science.gov (United States)

    Thompson, David W J; Bony, Sandrine; Li, Ying

    2017-08-01

    The troposphere is the region of the atmosphere characterized by low static stability, vigorous diabatic mixing, and widespread condensational heating in clouds. Previous research has argued that in the tropics, the upper bound on tropospheric mixing and clouds is constrained by the rapid decrease with height of the saturation water vapor pressure and hence radiative cooling by water vapor in clear-sky regions. Here the authors contend that the same basic physics play a key role in constraining the vertical structure of tropospheric mixing, tropopause temperature, and cloud-top temperature throughout the globe. It is argued that radiative cooling by water vapor plays an important role in governing the depth and amplitude of large-scale dynamics at extratropical latitudes.

  11. Characteristics and Mechanisms of Zonal Oscillation of Western Pacific Subtropical High in Summer

    Science.gov (United States)

    Guan, W.; Ren, X.; Hu, H.

    2017-12-01

    The zonal oscillation of the western Pacific subtropical high (WPSH) influences the weather and climate over East Asia significantly. This study investigates the features and mechanisms of the zonal oscillation of the WPSH during summer on subseasonal time scales. The zonal oscillation index of the WPSH is defined by normalized subseasonal geopotential height anomaly at 500hPa averaged over the WPSH's western edge (110° - 140°E, 10° - 30°N). The index shows a predominant oscillation with a period of 10-40 days. Large positive index indicates a strong anticyclonic anomaly over East Asia and its coastal region south of 30°N at both 850hPa and 500hPa. The WPSH stretches more westward accompanied by warmer SST anomalies beneath the western edge of the WPSH. Meanwhile, above-normal precipitation is seen over the Yangtze-Huaihe river basin and below-normal precipitation over the south of the Yangtze River. Negative index suggests a more eastward position of WPSH. The anomalies in circulation and SST for negative index are almost the mirror image of those for the positive index. In early summer, the zonal shift of the WPSH is affected by both the East Asia/Pacific (EAP) teleconnection pattern and the Silk road pattern (SRP). The positive (negative) phase of the EAP pattern is characterized by a low-level anticyclonic (cyclonic) anomaly over the subtropical western Pacific, indicating the western extension (eastward retreat) of the WPSH. Comparing with the EAP pattern, the SRP forms an upper-level anticyclonic (cyclonic) anomaly in mid-latitudes of East Asia, and then leads to the westward (eastward) movement of the WPSH. In late summer, the zonal shift of the WPSH is mainly affected by the EAP pattern, because the EAP pattern in late summer is stronger than that in early summer. The zonal shift of the WPSH is also influenced by the subseasonal air-sea interaction locally. During the early stage of WPSH's westward stretch, the local SST anomaly in late summer is

  12. ON THE VARIATION OF ZONAL GRAVITY COEFFICIENTS OF A GIANT PLANET CAUSED BY ITS DEEP ZONAL FLOWS

    International Nuclear Information System (INIS)

    Kong Dali; Zhang Keke; Schubert, Gerald

    2012-01-01

    Rapidly rotating giant planets are usually marked by the existence of strong zonal flows at the cloud level. If the zonal flow is sufficiently deep and strong, it can produce hydrostatic-related gravitational anomalies through distortion of the planet's shape. This paper determines the zonal gravity coefficients, J 2n , n = 1, 2, 3, ..., via an analytical method taking into account rotation-induced shape changes by assuming that a planet has an effective uniform density and that the zonal flows arise from deep convection and extend along cylinders parallel to the rotation axis. Two different but related hydrostatic models are considered. When a giant planet is in rigid-body rotation, the exact solution of the problem using oblate spheroidal coordinates is derived, allowing us to compute the value of its zonal gravity coefficients J-bar 2n , n=1,2,3,..., without making any approximation. When the deep zonal flow is sufficiently strong, we develop a general perturbation theory for estimating the variation of the zonal gravity coefficients, ΔJ 2n =J 2n -J-bar 2n , n=1,2,3,..., caused by the effect of the deep zonal flows for an arbitrarily rapidly rotating planet. Applying the general theory to Jupiter, we find that the deep zonal flow could contribute up to 0.3% of the J 2 coefficient and 0.7% of J 4 . It is also found that the shape-driven harmonics at the 10th zonal gravity coefficient become dominant, i.e., ΔJ 2n >=J-bar 2n for n ≥ 5.

  13. Tidal signatures of the thermospheric mass density and zonal wind at midlatitude: CHAMP and GRACE observations

    Directory of Open Access Journals (Sweden)

    C. Xiong

    2015-02-01

    Full Text Available By using the accelerometer measurements from CHAMP and GRACE satellites, the tidal signatures of the thermospheric mass density and zonal wind at midlatitudes have been analyzed in this study. The results show that the mass density and zonal wind at southern midlatitudes are dominated by a longitudinal wave-1 pattern. The most prominent tidal components in mass density and zonal wind are the diurnal tides D0 and DW2 and the semidiurnal tides SW1 and SW3. This is consistent with the tidal signatures in the F region electron density at midlatitudes as reported by Xiong and Lühr (2014. These same tidal components are observed both in the thermospheric and ionospheric quantities, supporting a mechanism that the non-migrating tides in the upper atmosphere are excited in situ by ion–neutral interactions at midlatitudes, consistent with the modeling results of Jones Jr. et al. (2013. We regard the thermospheric dynamics as the main driver for the electron density tidal structures. An example is the in-phase variation of D0 between electron density and mass density in both hemispheres. Further research including coupled atmospheric models is probably needed for explaining the similarities and differences between thermospheric and ionospheric tidal signals at midlatitudes.

  14. On the statistical connection between tropospheric and stratospheric circulation of the northern hemisphere in winter

    International Nuclear Information System (INIS)

    Perlwitz, J.; Graf, H.F.

    1994-01-01

    The associated anomaly patterns of the stratospheric geopotential height field and the tropospheric geopotential and temperature height fields of the northern hemisphere are determined applying the Canonical Correlation Analysis (CCA). With this linear multivariate technique the coupled modes of variability of time series of two fields are isolated in the EOF space. The one data set is the 50 hPa geopotential field, the other set consists of different height fields of the tropospheric pressure levels (200 hPa, 500 hPa, 700 hPa, 850 hPa) and the temperature of the 850 hPa pressure level. For the winter months (December, January, February) two natural coupled modes, a barotropic and a baroclinic one, of linear relationship between stratospheric and tropospheric circulation are found. The baroclinic mode describes a connection between the strength of the stratospheric cyclonic winter vortex and the tropospheric circulation over the North Atlantic. The corresponding temperature pattern for an anomalously strong stratospheric cyclonic vortex is characterized by positive temperature anomalies over higher latitudes of Eurasia. These 'Winter Warmings' are observed e.g. after violent volcanic eruptions. The barotropic mode is characterized by a zonal wave number one in the lower stratosphere and by a PNA-like pattern in the troposphere. It was shown by Labitzke and van Loon (1987) that this mode can be enhanced e.g. by El Ninos via the intensification of the Aleutian low. (orig.)

  15. Tropospheric Emission Spectrometer (TES) Data

    Data.gov (United States)

    National Aeronautics and Space Administration — TES focuses on the troposphere, the layer of atmosphere that stretches from the ground to the altitude at which airplanes fly. With very high spectral resolution,...

  16. Physics of the tropospheric radiopropagation

    International Nuclear Information System (INIS)

    Ajayi, G.O.

    1989-02-01

    The physics of the tropospheric radiopropagation is presented considering the atmospheric radio refractive index and taking into account the influence of precipitation and the attenuation due to the atmospheric gases. 35 refs, 20 figs, 3 tabs

  17. Transport in zonal flows in analogous geophysical and plasma systems

    Science.gov (United States)

    del-Castillo-Negrete, Diego

    1999-11-01

    Zonal flows occur naturally in the oceans and the atmosphere of planets. Important examples include the zonal flows in Jupiter, the stratospheric polar jet in Antarctica, and oceanic jets like the Gulf Stream. These zonal flows create transport barriers that have a crucial influence on mixing and confinement (e.g. the ozone depletion in Antarctica). Zonal flows also give rise to long-lasting vortices (e.g. the Jupiter red spot) by shear instability. Because of this, the formation and stability of zonal flows and their role on transport have been problems of great interest in geophysical fluid dynamics. On the other hand, zonal flows have also been observed in fusion plasmas and their impact on the reduction of transport has been widely recognized. Based on the well-known analogy between Rossby waves in quasigeostrophic flows and drift waves in magnetically confined plasmas, I will discuss the relevance to fusion plasmas of models and experiments recently developed in geophysical fluid dynamics. Also, the potential application of plasma physics ideas to geophysical flows will be discussed. The role of shear in the suppression of transport and the effect of zonal flows on the statistics of transport will be studied using simplified models. It will be shown how zonal flows induce large particle displacements that can be characterized as Lévy flights, and that the trapping effect of vortices combined with the zonal flows gives rise to anomalous diffusion and Lévy (non-Gaussian) statistics. The models will be compared with laboratory experiments and with atmospheric and oceanographic qualitative observations.

  18. Observing Tropospheric Ozone From Space

    Science.gov (United States)

    Fishman, Jack

    2000-01-01

    The importance of tropospheric ozone embraces a spectrum of relevant scientific issues ranging from local environmental concerns, such as damage to the biosphere and human health, to those that impact global change questions, Such is climate warming. From an observational perspective, the challenge is to determine the tropospheric ozone global distribution. Because its lifetime is short compared with other important greenhouse gases that have been monitored over the past several decades, the distribution of tropospheric ozone cannot be inferred from a relatively small set of monitoring stations. Therefore, the best way to obtain a true global picture is from the use of space-based instrumentation where important spatial gradients over vast ocean expanses and other uninhabited areas can be properly characterized. In this paper, the development of the capability to measure tropospheric ozone from space over the past 15 years is summarized. Research in the late 1980s successfully led to the determination of the climatology of tropospheric ozone as a function of season; more recently, the methodology has improved to the extent where regional air pollution episodes can be characterized. The most recent modifications now provide quasi-global (50 N) to 50 S) maps on a daily basis. Such a data set would allow for the study of long-range (intercontinental) transport of air pollution and the quantification of how regional emissions feed into the global tropospheric ozone budget. Future measurement capabilities within this decade promise to offer the ability to provide Concurrent maps of the precursors to the in situ formation of tropospheric ozone from which the scientific community will gain unprecedented insight into the processes that control global tropospheric chemistry

  19. Coherent Structure Phenomena in Drift Wave-Zonal Flow Turbulence

    International Nuclear Information System (INIS)

    Smolyakov, A. I.; Diamond, P. H.; Malkov, M.

    2000-01-01

    Zonal flows are azimuthally symmetric plasma potential perturbations spontaneously generated from small-scale drift-wave fluctuations via the action of Reynolds stresses. We show that, after initial linear growth, zonal flows can undergo further nonlinear evolution leading to the formation of long-lived coherent structures which consist of self-bound wave packets supporting stationary shear layers. Such coherent zonal flow structures constitute dynamical paradigms for intermittency in drift-wave turbulence that manifests itself by the intermittent distribution of regions with a reduced level of anomalous transport. (c) 2000 The American Physical Society

  20. The Role of Subtropical Irreversible PV Mixing in the Zonal Mean Circulation Response to Global Warming-like Thermal Forcing

    Energy Technology Data Exchange (ETDEWEB)

    Lu, Jian [Pacific Northwest National Lab. (PNNL), Richland, WA (United States); Sun, Lantao [National Center for Atmospheric Research, Boulder, CO (United States); Wu, Yutian [New York Univ. (NYU), NY (United States); Chen, Gang [Cornell Univ., Ithaca, NY (United States)

    2013-11-21

    The atmospheric circulation response to the global warming-like tropical upper tropospheric heating is revisited using a dry atmospheric general circulation model (AGCM) in light of a new diagnostics based on the concept of finite-amplitude wave activity (FAWA) on equivalent latitude. For a given tropical heating profile, the linear Wentzel-Kramers-Brillouin (WKB) wave refraction analysis sometimes gives a very different and even opposite prediction of the eddy momentum flux response to that of the actual full model simulation, exposing the limitation of the traditional linear approach in understanding the full dynamics of the atmospheric response under global warming. The implementation of the FAWA diagnostics reveals that in response to the upper tropospheric heating, effective diffusivity, a measure of the mixing efficiency, increases and advances upward and poleward in the subtropics and the resultant enhancement and the poleward encroachment of eddy potential vorticity mixing leads to a poleward displaced potential vorticity (PV) gradient peak in the upper troposphere. The anomalous eddy PV flux, in balance with the PV dissipation, gives rise to a poleward shift in the eddy-driven jet and eddy-driven mean meridional circulation. Sensitivity experiments show that these irreversible dissipation processes in the upper troposphere are robust, regardless of the width of the tropical heating.

  1. Source attribution of tropospheric ozone

    Science.gov (United States)

    Butler, T. M.

    2015-12-01

    Tropospheric ozone is a harmful pollutant with adverse effects on human health and ecosystems. As well as these effects, tropospheric ozone is also a powerful greenhouse gas, with an anthropogenic radiative forcing one quarter of that of CO2. Along with methane and atmospheric aerosol, tropospheric ozone belongs to the so-called Short Lived Climate forcing Pollutants, or SLCP. Recent work has shown that efforts to reduce concentrations of SLCP in the atmosphere have the potential to slow the rate of near-term climate change, while simultaneously improving public health and reducing crop losses. Unlike many other SLCP, tropospehric ozone is not directly emitted, but is instead influenced by two distinct sources: transport of air from the ozone-rich stratosphere; and photochemical production in the troposphere from the emitted precursors NOx (oxides of nitrogen), CO (Carbon Monoxide), and VOC (volatile organic compounds, including methane). Better understanding of the relationship between ozone production and the emissions of its precursors is essential for the development of targeted emission reduction strategies. Several modeling methods have been employed to relate the production of tropospheric ozone to emissions of its precursors; emissions perturbation, tagging, and adjoint sensitivity methods all deliver complementary information about modelled ozone production. Most studies using tagging methods have focused on attribution of tropospheric ozone production to emissions of NOx, even though perturbation methods have suggested that tropospheric ozone is also sensitive to VOC, particularly methane. In this study we describe the implementation into a global chemistry-climate model of a scheme for tagging emissions of NOx and VOC with an arbitrary number of labels, which are followed through the chemical reactions of tropospheric ozone production in order to perform attribution of tropospehric ozone to its emitted precursors. Attribution is performed to both

  2. Photoreceptor atrophy in acute zonal occult outer retinopathy

    DEFF Research Database (Denmark)

    Zibrandtsen, N.; Munch, I.C.; Klemp, K.

    2006-01-01

    Purpose: To assess retinal morphology in acute zonal occult outer retinopathy (AZOOR). Methods: Three patients with a normal ophthalmoscopic fundus appearance, a history of photopsia, and visual field loss compatible with AZOOR were examined using optical coherence tomography, automated perimetry...

  3. Zonal flow generation in collisionless trapped electron mode turbulence

    International Nuclear Information System (INIS)

    Anderson, J; Nordman, H; Singh, R; Weiland, J

    2006-01-01

    In the present work the generation of zonal flows in collisionless trapped electron mode (TEM) turbulence is studied analytically. A reduced model for TEM turbulence is utilized based on an advanced fluid model for reactive drift waves. An analytical expression for the zonal flow growth rate is derived and compared with the linear TEM growth, and its scaling with plasma parameters is examined for typical tokamak parameter values

  4. Tokamak residual zonal flow level in near-separatrix region

    International Nuclear Information System (INIS)

    Bing-Ren, Shi

    2010-01-01

    Residual zonal flow level is calculated for tokamak plasmas in the near-separatrix region of a diverted tokamak. A recently developed method is used to construct an analytic divertor tokamak configuration. It is shown that the residual zonal flow level becomes smaller but still keeps finite near the separatrix because the neoclassical polarisation mostly due to the trapped particles goes larger in this region. (fluids, plasmas and electric discharges)

  5. Zonal Flow Dynamics and Size-scaling of Anomalous Transport

    International Nuclear Information System (INIS)

    Liu Chen; White, Roscoe B.; Zonca, F.

    2003-01-01

    Nonlinear equations for the slow space-time evolution of the radial drift wave envelope and zonal flow amplitude have been self-consistently derived for a model nonuniform tokamak equilibrium within the coherent 4-wave drift wave-zonal flow modulation interaction model of Chen, Lin, and White [Phys. Plasmas 7 (2000) 3129]. Solutions clearly demonstrate turbulence spreading due to nonlinearly enhanced dispersiveness and, consequently, the device-size dependence of the saturated wave intensities and transport coefficients

  6. Transport hysteresis and zonal flow stimulation in magnetized plasmas

    Science.gov (United States)

    Gravier, E.; Lesur, M.; Reveille, T.; Drouot, T.; Médina, J.

    2017-12-01

    A hysteresis in the relationship between zonal flows and electron heating is observed numerically by using gyrokinetic simulations in fusion plasmas. As the electron temperature increases, a first transition occurs, at a given electron/ion temperature ratio, above which zonal flows are much weaker than before the transition, leading to a poorly confined plasma. Beyond this transition, even if the electron temperature is lowered to a moderate value, the plasma fails to recover a dynamic state with strong zonal flows. Then, as the electron temperature decreases further, a new transition appears, at a temperature lower than the first transition, below which the zonal flows are stronger than they were initially. The confinement of the plasma and the heat flux are thus found to be sensitive to the history of the magnetized plasma. These transitions are associated with large exchanges of energy between the modes corresponding to instabilities ( m> 0 ) and zonal flows ( m = 0 ). We also observe that up to the first transition it is possible to use a control method to stimulate the appearance of zonal flows and therefore the confinement of the plasma. Beyond that transition, this control method is no longer effective.

  7. The Governing Processes and Timescales of Stratosphere-to-Troposphere Transport and its Contribution to Ozone in the Arctic Troposphere

    Science.gov (United States)

    Liang, Q.; Douglass, A. R.; Duncan, B. N.; Stolarski, R. S.; Witte, J. C.

    2009-01-01

    We used the seasonality of a combination of atmospheric trace gases and idealized tracers to examine stratosphere-to-troposphere transport and its influence on tropospheric composition in the Arctic. Maximum stratosphere-to-troposphere transport of CFCs and O3 occurs in April as driven by the Brewer-Dobson circulation. Stratosphere-troposphere exchange (STE) occurs predominantly between 40 deg N to 80 deg N with stratospheric influx in the mid-latitudes (30-70 deg N) accounting for 67.81 percent of the air of stratospheric origin in the Northern Hemisphere extratropical troposphere. Transport from the lower stratosphere to the lower troposphere (LT) takes three months on average, one month to cross the tropopause, the second month to travel from the upper troposphere (UT) to the middle troposphere (MT), and the third month to reach the LT. During downward transport, the seasonality of a trace gas can be greatly impacted by wet removal and chemistry. A comparison of idealized tracers with varying lifetimes suggests that when initialized with the same concentrations and seasonal cycles at the tropopause, trace gases that have shorter lifetimes display lower concentrations, smaller amplitudes, and earlier seasonal maxima during transport to the LT. STE contributes to O3 in the Arctic troposphere directly from the transport of O3 and indirectly from the transport of NOy . Direct transport of O3 from the stratosphere accounts for 78 percent of O3 in the Arctic UT with maximum contributions occurring from March to May. The stratospheric contribution decreases significantly in the MT/LT (20.25 percent of total O3) and shows a very weak March.April maximum. Our NOx budget analysis in the Arctic UT shows that during spring and summer, the stratospheric injection of NO y-rich air increases NOx concentrations above the 20 pptv threshold level, thereby shifting the Arctic UT from a regime of net photochemical ozone loss to one of net production with rates as high as +16 ppbv/month.

  8. The transformation of vegetation vertical zonality affected by anthropogenic impact in East Fennoscandia (Russia)

    Science.gov (United States)

    Sidorik, Vadim; Miulgauzen, Daria

    2017-04-01

    Ecosystems of East Fennoscandia have been affected by intensive anthropogenic influence that resulted in their significant transformation. Study of ecosystems in the framework of vegetation vertical zonality disturbance as well as its recovery allows to understand the trends of anthropogenically induced changes. The aim of the present research is the comparative analysis of vegetation vertical zonality of the two uplands in East Fennoscandia which may be considered as unaffected and affected by anthropogenic impact. The objects of key studies carried out in the north-west of Kola Peninsula in the vicinity of the Pechenganikel Mining and Metallurgical Plant are represented by ecosystems of Kalkupya (h 357 m) and Hangaslachdenvara (h 284 m) uplands. They are characterized by the similarity in sequence of altitudinal belts due to the position on the northern taiga - forest-tundra boundary. Plant communities of Kalkupya upland have no visible signs of anthropogenic influence, therefore, they can be considered as model ecosystems of the area. The sequence of altitudinal belts is the following: - up to 200 m - pine subshrub and green moss ("zonal") forest replaced by mixed pine and birch forest near the upper boundary; - 200-300 m - birch crooked subshrub wood; - above 300 m - tundra subshrub and lichen communities. Ecosystems of Hangaslachdenvara upland have been damaged by air pollution (SO2, Ni, Cu emissions) of the Pechenganikel Plant. This impact has led to plant community suppression and formation of barren lands. Besides the soil cover was significantly disturbed, especially upper horizons. Burying of soil profiles, represented by Podzols (WRB, 2015), also manifested itself in the exploited part of the area. The vegetation cover of Hangaslachdenvara upland is the following: - up to 130 m - birch and aspen subshrub and grass forest instead of pine forest ("zonal"); - 130-200 m - barren lands instead of pine forest ("zonal"); - above 200 m - barren lands instead of

  9. The meteorological environment of the tropospheric ozone maximum over the tropical South Atlantic

    Energy Technology Data Exchange (ETDEWEB)

    Krishnamurti, T N; Fuelberg, H E; Bensman, E L; Sinha, M C; Oosterhof, D; Kumar, V B [Florida State University, Tallahassee, FL (United States). Department of Meteorology

    1993-01-01

    This paper examines atmospheric flow patterns over the Southern Atlantic Ocean, where a maximum of tropospheric ozone is observed just west of Southern Africa. The climatology of the South Atlantic basin is shown to favour flow off from South America and Africa converging into the area of high tropospheric ozone. This ozone is initially attributable to byproducts of biomass burning over both these continents. A case study, carried out over 6 days during October 1989, was used to determine the effect of a purely advective scheme (no photochemistry) on the distribution of ozone over the basin. The results showed a pattern in which ozone accumulated off the west coast of South Africa within 72 hours after beginning with an homogenous, zonally-symmetric distribution of ozone. 11 refs.

  10. Tropospheric ozone annual variation and possible troposphere-stratosphere coupling in the Arctic and Antarctic as derived from ozone soundings at Resolute and Amundsen-Scott stations

    Energy Technology Data Exchange (ETDEWEB)

    Gruzdev, A.N.; Sitnov, S.A. (Russian Academy of Sciences, Moscow (Russian Federation). Inst. of Atmospheric Physics)

    1993-01-01

    The tropospheric ozone annual variation in the northern and southern polar regions is analyzed from ozone sounding data obtained at Resolute during a 15-year period and Amundsen-Scott during a 7-year period. The phase of ozone annual variation above Resolute changes (increases) gradually from the stratosphere across the tropopause to the middle troposphere. Unlike this, the phase of the Antarctic ozone annual harmonic has a discontinuity in the layer of the changing tropopause level, so that the annual harmonic in the upper troposphere, lower stratosphere is 4-to-5 months out of phase (earlier) to that above and beneath. Above both the Arctic and Antarctic stations, the ozone mixing ratio and its vertical gradient evolve in a similar manner in the wide layer from the lower stratosphere to the middle troposphere. This likely points out that ozone in this layer is controlled from above. An indication of the stratospheric-tropospheric ozone exchange above Resolute is noted from mid-winter to spring. The analysis of columnar tropospheric ozone changes gives a lower estimate of the cross-tropopause ozone flux up to 5x10[sup 10] mol cm[sup -2] s[sup -1]. Above the South Pole, the cross-tropopause ozone flux is not usually large. There is also some evidence that early in the spring, when the stratospheric ozone 'hole' is developed, the stratospheric-tropospheric exchange conducts the influence of the 'hole' into the upper troposphere, where the integrated ozone destruction is estimated to be 8x10[sup 10] mol cm[sup -2] s[sup -1]. Correlation analysis gives no ozone-tropopause correlation in the Antarctic in winter, while in other seasons as well as during all seasons in the Arctic, there are negative correlation peaks just above the tropopause. (19 refs., 6 figs.).

  11. Ozone zonal asymmetry and planetary wave characterization during Antarctic spring

    Directory of Open Access Journals (Sweden)

    I. Ialongo

    2012-03-01

    Full Text Available A large zonal asymmetry of ozone has been observed over Antarctica during winter-spring, when the ozone hole develops. It is caused by a planetary wave-driven displacement of the polar vortex. The total ozone data by OMI (Ozone Monitoring Instrument and the ozone profiles by MLS (Microwave Limb Sounder and GOMOS (Global Ozone Monitoring by Occultation of Stars were analysed to characterize the ozone zonal asymmetry and the wave activity during Antarctic spring. Both total ozone and profile data have shown a persistent zonal asymmetry over the last years, which is usually observed from September to mid-December. The largest amplitudes of planetary waves at 65° S (the perturbations can achieve up to 50% of zonal mean values is observed in October. The wave activity is dominated by the quasi-stationary wave 1 component, while the wave 2 is mainly an eastward travelling wave. Wave numbers 1 and 2 generally explain more than the 90% of the ozone longitudinal variations. Both GOMOS and MLS ozone profile data show that ozone zonal asymmetry covers the whole stratosphere and extends up to the altitudes of 60–65 km. The wave amplitudes in ozone mixing ratio decay with altitude, with maxima (up to 50% below 30 km.

    The characterization of the ozone zonal asymmetry has become important in the climate research. The inclusion of the polar zonal asymmetry in the climate models is essential for an accurate estimation of the future temperature trends. This information might also be important for retrieval algorithms that rely on ozone a priori information.

  12. Remote sensed and in situ constraints on processes affecting tropical tropospheric ozone

    Directory of Open Access Journals (Sweden)

    B. Sauvage

    2007-01-01

    Full Text Available We use a global chemical transport model (GEOS-Chem to evaluate the consistency of satellite measurements of lightning flashes and ozone precursors with in situ measurements of tropical tropospheric ozone. The measurements are tropospheric O3, NO2, and HCHO columns from the GOME satellite instrument, lightning flashes from the OTD and LIS satellite instruments, profiles of O3, CO, and relative humidity from the MOZAIC aircraft program, and profiles of O3 from the SHADOZ ozonesonde network. We interpret these multiple data sources with our model to better understand what controls tropical tropospheric ozone. Tropical tropospheric ozone is mainly affected by lightning NOx and convection in the upper troposphere and by surface emissions in the lower troposphere. Scaling the spatial distribution of lightning in the model to the observed flashes improves the simulation of O3 in the upper troposphere by 5–20 ppbv versus in situ observations and by 1–4 Dobson Units versus GOME retrievals of tropospheric O3 columns. A lightning source strength of 6±2 Tg N/yr best represents in situ observations from aircraft and ozonesonde. Tropospheric NO2 and HCHO columns from GOME are applied to provide top-down constraints on emission inventories of NOx (biomass burning and soils and VOCs (biomass burning. The top-down biomass burning inventory is larger than the bottom-up inventory by a factor of 2 for HCHO and alkenes, and by a factor of 2.6 for NOx over northern equatorial Africa. These emissions increase lower tropospheric O3 by 5–20 ppbv, improving the simulation versus aircraft observations, and by 4 Dobson Units versus GOME observations of tropospheric O3 columns. Emission factors in the a posteriori inventory are more consistent with a recent compilation from in situ measurements. The ozone simulation using two different dynamical schemes (GEOS-3 and GEOS-4 is evaluated versus observations; GEOS-4 better represents O3 observations by 5–15 ppbv

  13. Numerical Simulation on Zonal Disintegration in Deep Surrounding Rock Mass

    Directory of Open Access Journals (Sweden)

    Xuguang Chen

    2014-01-01

    Full Text Available Zonal disintegration have been discovered in many underground tunnels with the increasing of embedded depth. The formation mechanism of such phenomenon is difficult to explain under the framework of traditional rock mechanics, and the fractured shape and forming conditions are unclear. The numerical simulation was carried out to research the generating condition and forming process of zonal disintegration. Via comparing the results with the geomechanical model test, the zonal disintegration phenomenon was confirmed and its mechanism is revealed. It is found to be the result of circular fracture which develops within surrounding rock mass under the high geostress. The fractured shape of zonal disintegration was determined, and the radii of the fractured zones were found to fulfill the relationship of geometric progression. The numerical results were in accordance with the model test findings. The mechanism of the zonal disintegration was revealed by theoretical analysis based on fracture mechanics. The fractured zones are reportedly circular and concentric to the cavern. Each fracture zone ruptured at the elastic-plastic boundary of the surrounding rocks and then coalesced into the circular form. The geometric progression ratio was found to be related to the mechanical parameters and the ground stress of the surrounding rocks.

  14. Numerical simulation on zonal disintegration in deep surrounding rock mass.

    Science.gov (United States)

    Chen, Xuguang; Wang, Yuan; Mei, Yu; Zhang, Xin

    2014-01-01

    Zonal disintegration have been discovered in many underground tunnels with the increasing of embedded depth. The formation mechanism of such phenomenon is difficult to explain under the framework of traditional rock mechanics, and the fractured shape and forming conditions are unclear. The numerical simulation was carried out to research the generating condition and forming process of zonal disintegration. Via comparing the results with the geomechanical model test, the zonal disintegration phenomenon was confirmed and its mechanism is revealed. It is found to be the result of circular fracture which develops within surrounding rock mass under the high geostress. The fractured shape of zonal disintegration was determined, and the radii of the fractured zones were found to fulfill the relationship of geometric progression. The numerical results were in accordance with the model test findings. The mechanism of the zonal disintegration was revealed by theoretical analysis based on fracture mechanics. The fractured zones are reportedly circular and concentric to the cavern. Each fracture zone ruptured at the elastic-plastic boundary of the surrounding rocks and then coalesced into the circular form. The geometric progression ratio was found to be related to the mechanical parameters and the ground stress of the surrounding rocks.

  15. The role of zonal flows in disc gravito-turbulence

    Science.gov (United States)

    Vanon, R.

    2018-04-01

    The work presented here focuses on the role of zonal flows in the self-sustenance of gravito-turbulence in accretion discs. The numerical analysis is conducted using a bespoke pseudo-spectral code in fully compressible, non-linear conditions. The disc in question, which is modelled using the shearing sheet approximation, is assumed to be self-gravitating, viscous, and thermally diffusive; a constant cooling timescale is also considered. Zonal flows are found to emerge at the onset of gravito-turbulence and they remain closely linked to the turbulent state. A cycle of zonal flow formation and destruction is established, mediated by a slow mode instability (which allows zonal flows to grow) and a non-axisymmetric instability (which disrupts the zonal flow), which is found to repeat numerous times. It is in fact the disruptive action of the non-axisymmetric instability to form new leading and trailing shearing waves, allowing energy to be extracted from the background flow and ensuring the self-sustenance of the gravito-turbulent regime.

  16. The role of zonal flows in disc gravito-turbulence

    Science.gov (United States)

    Vanon, R.

    2018-07-01

    The work presented here focuses on the role of zonal flows in the self-sustenance of gravito-turbulence in accretion discs. The numerical analysis is conducted using a bespoke pseudo-spectral code in fully compressible, non-linear conditions. The disc in question, which is modelled using the shearing sheet approximation, is assumed to be self-gravitating, viscous, and thermally diffusive; a constant cooling time-scale is also considered. Zonal flows are found to emerge at the onset of gravito-turbulence and they remain closely linked to the turbulent state. A cycle of zonal flow formation and destruction is established, mediated by a slow mode instability (which allows zonal flows to grow) and a non-axisymmetric instability (which disrupts the zonal flow), which is found to repeat numerous times. It is in fact the disruptive action of the non-axisymmetric instability to form new leading and trailing shearing waves, allowing energy to be extracted from the background flow and ensuring the self-sustenance of the gravito-turbulent regime.

  17. Solar-cycle variation of zonal and meridional flow

    International Nuclear Information System (INIS)

    Komm, R; Howe, R; Hill, F; Hernandez, I Gonzalez; Haber, D

    2011-01-01

    We study the variation with the solar cycle of the zonal and meridional flows in the near-surface layers of the solar convection zone. We have analyzed MDI Dynamics-Program data with ring-diagram analysis covering the rising phase of cycle 23, while the analyzed GONG high-resolution data cover the maximum and declining phase of cycle 23. For the zonal flow, the migration with latitude of the flow pattern is apparent in the deeper layers, while for the meridional flow, a migration with latitude is apparent only in the layers close to the surface. The faster-than-average bands of the zonal flow associated with the new cycle are clearly visible. Similarly, a pattern related to the new cycle appears in the residual meridional flow. We also study the flow differences between the hemispheres during the course of the solar cycle. The difference pattern of the meridional flow is slanted in latitude straddling the faster-than-average band of the torsional oscillation pattern in the zonal flow. The difference pattern of the zonal flow, on the other hand, resembles the cycle variation of the meridional flow. In addition, the meridional flow during the minimum of cycle 23/24 appears to be slightly stronger than during the previous minimum of cycle 22/23.

  18. First Directly Retrieved Global Distribution of Tropospheric Column Ozone from GOME: Comparison with the GEOS-CHEM Model

    Science.gov (United States)

    Liu, Xiong; Chance, Kelly; Sioris, Christopher E.; Kurosu, Thomas P.; Spurr, Robert J. D.; Martin, Randall V.; Fu, Tzung-May; Logan, Jennifer A.; Jacob, Daniel J.; Palmer, Paul I.; hide

    2006-01-01

    We present the first directly retrieved global distribution of tropospheric column ozone from Global Ozone Monitoring Experiment (GOME) ultraviolet measurements during December 1996 to November 1997. The retrievals clearly show signals due to convection, biomass burning, stratospheric influence, pollution, and transport. They are capable of capturing the spatiotemporal evolution of tropospheric column ozone in response to regional or short time-scale events such as the 1997-1998 El Nino event and a 10-20 DU change within a few days. The global distribution of tropospheric column ozone displays the well-known wave-1 pattern in the tropics, nearly zonal bands of enhanced tropospheric column ozone of 36-48 DU at 20degS-30degS during the austral spring and at 25degN-45degN during the boreal spring and summer, low tropospheric column ozone of 33 DU at some northern high-latitudes during the spring. Simulation from a chemical transport model corroborates most of the above structures, with small biases of <+/-5 DU and consistent seasonal cycles in most regions, especially in the southern hemisphere. However, significant positive biases of 5-20 DU occur in some northern tropical and subtropical regions such as the Middle East during summer. Comparison of GOME with monthly-averaged Measurement of Ozone and Water Vapor by Airbus in-service Aircraft (MOZAIC) tropospheric column ozone for these regions usually shows good consistency within 1 a standard deviations and retrieval uncertainties. Some biases can be accounted for by inadequate sensitivity to lower tropospheric ozone, the different spatiotemporal sampling and the spatiotemporal variations in tropospheric column ozone.

  19. Ozone in the Tropical Troposphere

    NARCIS (Netherlands)

    Peters, Wouter

    2002-01-01

    The aim of the research presented here is to acquire knowledge of the past, present, and future composition, stability, sensitivity, and variability of the troposphere. We focus mostly on the tropical regions because it has received little attention so far, measurements here are scarce, and large

  20. Overview of edge turbulence and zonal flow studies on TEXTOR

    International Nuclear Information System (INIS)

    Xu, Y.; Kraemer-Flecken, A.; Reiser, D.

    2008-01-01

    In the TEXTOR tokamak, the edge turbulence properties and turbulence-associated zonal flows have been systematically investigated both experimentally and theoretically. The experimental results include the investigation of self-organized criticality (SOC) behavior, the intermittent blob transport and the geodesic acoustic mode (GAM) zonal flows. During the Dynamic Ergodic Divertor (DED) operation in TEXTOR, the impact of an ergodized plasma boundary on edge turbulence, turbulent transport and the fluctuation propagation has also been studied in detail. The results show substantial influence by the DED on edge turbulence. The theoretical simulations for TEXTOR parameters show characteristic features of the GAM flows and strong reduction of the blob transport by the DED at the plasma periphery. Moreover, the modelling reveals the importance of the Reynolds stress in driving mean (or zonal) flows at the plasma edge in the ohmic discharge phase in TEXTOR. (author)

  1. Influence of the Gulf Stream on the troposphere.

    Science.gov (United States)

    Minobe, Shoshiro; Kuwano-Yoshida, Akira; Komori, Nobumasa; Xie, Shang-Ping; Small, Richard Justin

    2008-03-13

    The Gulf Stream transports large amounts of heat from the tropics to middle and high latitudes, and thereby affects weather phenomena such as cyclogenesis and low cloud formation. But its climatic influence, on monthly and longer timescales, remains poorly understood. In particular, it is unclear how the warm current affects the free atmosphere above the marine atmospheric boundary layer. Here we consider the Gulf Stream's influence on the troposphere, using a combination of operational weather analyses, satellite observations and an atmospheric general circulation model. Our results reveal that the Gulf Stream affects the entire troposphere. In the marine boundary layer, atmospheric pressure adjustments to sharp sea surface temperature gradients lead to surface wind convergence, which anchors a narrow band of precipitation along the Gulf Stream. In this rain band, upward motion and cloud formation extend into the upper troposphere, as corroborated by the frequent occurrence of very low cloud-top temperatures. These mechanisms provide a pathway by which the Gulf Stream can affect the atmosphere locally, and possibly also in remote regions by forcing planetary waves. The identification of this pathway may have implications for our understanding of the processes involved in climate change, because the Gulf Stream is the upper limb of the Atlantic meridional overturning circulation, which has varied in strength in the past and is predicted to weaken in response to human-induced global warming in the future.

  2. A model study of ozone in the eastern Mediterranean free troposphere during MINOS (August 2001

    Directory of Open Access Journals (Sweden)

    G. J. Roelofs

    2003-01-01

    Full Text Available A coupled tropospheric chemistry-climate model is used to analyze tropospheric ozone distributions observed during the MINOS campaign in the eastern Mediterranean region (August, 2001. Modeled ozone profiles are generally in good agreement with the observations. Our analysis shows that the atmospheric dynamics in the region are strongly influenced by the occurrence of an upper tropospheric anti-cyclone, associated with the Asian summer monsoon and centered over the Tibetan Plateau. The anti-cyclone affects the chemical composition of the upper troposphere, where ozone concentrations of about 50 ppbv were measured, through advection of boundary layer air from South-East Asia. A layer between 4-6 km thickness was present beneath, containing up to 120 ppbv of ozone with substantial contributions by transport from the stratosphere and through lightning NOx. Additionally, pollutant ozone from North America was mixed in. Ozone in the lower troposphere originated mainly from the European continent. The stratospheric influence may be overestimated due to too strong vertical diffusion associated with the relatively coarse vertical resolution. The estimated tropospheric ozone column over the eastern Mediterranean is ~50 DU in summer, to which ozone from recent stratospheric origin contributes about 30%, ozone from lightning 13%, and from South-East Asia, North America and Europe about 7%, 8% and 14%, respectively, adding to a long-term hemispheric background of 25% of the column.

  3. Rethinking wave-kinetic theory applied to zonal flows

    Science.gov (United States)

    Parker, Jeffrey

    2017-10-01

    Over the past two decades, a number of studies have employed a wave-kinetic theory to describe fluctuations interacting with zonal flows. Recent work has uncovered a defect in this wave-kinetic formulation: the system is dominated by the growth of (arbitrarily) small-scale zonal structures. Theoretical calculations of linear growth rates suggest, and nonlinear simulations confirm, that this system leads to the concentration of zonal flow energy in the smallest resolved scales, irrespective of the numerical resolution. This behavior results from the assumption that zonal flows are extremely long wavelength, leading to the neglect of key terms responsible for conservation of enstrophy. A corrected theory, CE2-GO, is presented; it is free of these errors yet preserves the intuitive phase-space mathematical structure. CE2-GO properly conserves enstrophy as well as energy, and yields accurate growth rates of zonal flow. Numerical simulations are shown to be well-behaved and not dependent on box size. The steady-state limit simplifies into an exact wave-kinetic form which offers the promise of deeper insight into the behavior of wavepackets. The CE2-GO theory takes its place in a hierarchy of models as the geometrical-optics reduction of the more complete cumulant-expansion statistical theory CE2. The new theory represents the minimal statistical description, enabling an intuitive phase-space formulation and an accurate description of turbulence-zonal flow dynamics. This work was supported by an NSF Graduate Research Fellowship, a US DOE Fusion Energy Sciences Fellowship, and US DOE Contract Nos. DE-AC52-07NA27344 and DE-AC02-09CH11466.

  4. Ozone variability in the troposphere and the stratosphere from the first 6 years of IASI observations (2008–2013

    Directory of Open Access Journals (Sweden)

    C. Wespes

    2016-05-01

    Full Text Available In this paper, we assess how daily ozone (O3 measurements from the Infrared Atmospheric Sounding Interferometer (IASI on the MetOp-A platform can contribute to the analyses of the processes driving O3 variability in the troposphere and the stratosphere and, in the future, to the monitoring of long-term trends. The temporal evolution of O3 during the first 6 years of IASI (2008–2013 operation is investigated with multivariate regressions separately in four different layers (ground–300, 300–150, 150–25, 25–3 hPa, by adjusting to the daily time series averaged in 20° zonal bands, seasonal and linear trend terms along with important geophysical drivers of O3 variation (e.g. solar flux, quasi-biennial oscillation (QBO. The regression model is shown to perform generally very well with a strong dominance of the annual harmonic terms and significant contributions from O3 drivers, in particular in the equatorial region where the QBO and the solar flux contribution dominate. More particularly, despite the short period of the IASI data set available up to now, two noticeable statistically significant apparent trends are inferred from the daily IASI measurements: a positive trend in the upper stratosphere (e.g. 1.74 ± 0.77 DU year−1 between 30 and 50° S, which is consistent with other studies suggesting a turnaround for stratospheric O3 recovery, and a negative trend in the troposphere at the mid-latitudes and high northern latitudes (e.g. −0.26 ± 0.11 DU year−1 between 30 and 50° N, especially during summer and probably linked to the impact of decreasing ozone precursor emissions. The impact of the high temporal sampling of IASI on the uncertainty in the determination of O3 trend has been further explored by performing multivariate regressions on IASI monthly averages and on ground-based Fourier transform infrared (FTIR measurements.

  5. Medium-range mid-tropospheric transport of ozone and precursors over Africa: two numerical case studies in dry and wet seasons

    Directory of Open Access Journals (Sweden)

    B. Sauvage

    2007-10-01

    Full Text Available A meso-scale model was used to understand and describe the dynamical processes driving high ozone concentrations observed during both dry and monsoon season in monthly climatologies profiles over Lagos (Nigeria, 6.6° N, 3.3° E, obtained with the MOZAIC airborne measurements (ozone and carbon monoxide. This study focuses on ozone enhancements observed in the upper-part of the lower troposphere, around 3000 m. Two individual cases have been selected in the MOZAIC dataset as being representative of the climatological ozone enhancements, to be simulated and analyzed with on-line Lagrangian backtracking of air masses.

    This study points out the role of baroclinic low-level circulations present in the Inter Tropical Front (ITF area. Two low-level thermal cells around a zonal axis and below 2000 m, in mirror symmetry to each other with respect to equator, form near 20° E and around 5° N and 5° S during the (northern hemisphere dry and wet seasons respectively. They are caused by surface gradients – the warm dry surface being located poleward of the ITF and the cooler wet surface equatorward of the ITF.

    A convergence line exists between the poleward low-level branch of each thermal cell and the equatorward low-level branch of the Hadley cell. Our main conclusion is to point out this line as a preferred location for fire products – among them ozone precursors – to be uplifted and injected into the lower free troposphere.

    The free tropospheric transport that occurs then depends on the hemisphere and season. In the NH dry season, the AEJ allows transport of ozone and precursors westward to Lagos. In the NH monsoon (wet season, fire products are transported from the southern hemisphere to Lagos by the southeasterly trade that surmounts the monsoon layer. Additionally ozone precursors uplifted by wet convection in the ITCZ can also mix to the ones uplifted by the baroclinic cell and be advected up to Lagos by the trade

  6. Daily estimates of the migrating tide and zonal mean temperature in the mesosphere and lower thermosphere derived from SABER data

    Science.gov (United States)

    Ortland, David A.

    2017-04-01

    Satellites provide a global view of the structure in the fields that they measure. In the mesosphere and lower thermosphere, the dominant features in these fields at low zonal wave number are contained in the zonal mean, quasi-stationary planetary waves, and tide components. Due to the nature of the satellite sampling pattern, stationary, diurnal, and semidiurnal components are aliased and spectral methods are typically unable to separate the aliased waves over short time periods. This paper presents a data processing scheme that is able to recover the daily structure of these waves and the zonal mean state. The method is validated by using simulated data constructed from a mechanistic model, and then applied to Sounding of the Atmosphere using Broadband Emission Radiometry (SABER) temperature measurements. The migrating diurnal tide extracted from SABER temperatures for 2009 has a seasonal variability with peak amplitude (20 K at 95 km) in February and March and minimum amplitude (less than 5 K at 95 km) in early June and early December. Higher frequency variability includes a change in vertical structure and amplitude during the major stratospheric warming in January. The migrating semidiurnal tide extracted from SABER has variability on a monthly time scale during January through March, minimum amplitude in April, and largest steady amplitudes from May through September. Modeling experiments were performed that show that much of the variability on seasonal time scales in the migrating tides is due to changes in the mean flow structure and the superposition of the tidal responses to water vapor heating in the troposphere and ozone heating in the stratosphere and lower mesosphere.

  7. Intermittent characteristics in coupling between turbulence and zonal flows

    International Nuclear Information System (INIS)

    Fujisawa, A; Shimizu, A; Nakano, H; Ohshima, S; Itoh, K; Nagashima, Y; Itoh, S-I; Iguchi, H; Yoshimura, Y; Minami, T; Nagaoka, K; Takahashi, C; Kojima, M; Nishimura, S; Isobe, M; Suzuki, C; Akiyama, T; Ido, T; Matsuoka, K; Okamura, S; Diamond, P H

    2007-01-01

    An extended application of Gabour's wavelet to bicoherence analysis succeeds in resolving the instantaneous structure of three wave couplings between disparate scale electric field fluctuations in the high temperature core in a toroidal plasma device named the compact helical system. The obtained results quantify an intermittent linkage between turbulence and zonal flows-a highlighted issue in the present plasma research. This is the first demonstration that the intermittent nature of the three wave coupling should underlie the turbulence power modulation due to zonal flows

  8. Nongeostrophic theory of zonally averaged circulation. I - Formulation

    Science.gov (United States)

    Tung, Ka Kit

    1986-01-01

    A nongeostrophic theory of zonally averaged circulation is formulated using the nonlinear primitive equations (mass conservation, thermodynamics, and zonal momentum) on a sphere. The relationship between the mean meridional circulation and diabatic heating rate is studied. Differences between results of nongeostropic theory and the geostrophic formulation concerning the role of eddy forcing of the diabatic circulation and the nonlinear nearly inviscid limit versus the geostrophic limit are discussed. Consideration is given to the Eliassen-Palm flux divergence, the Eliassen-Palm pseudodivergence, the nonacceleration theorem, and the nonlinear nongeostrophic Taylor relationship.

  9. Characterization of zonal flow generation in weak electrostatic turbulence

    International Nuclear Information System (INIS)

    Negrea, M; Petrisor, I; Weyssow, B

    2008-01-01

    The influence of the diamagnetic Kubo number, which is proportional to the diamagnetic drift velocity, on the zonal flow generation by an anisotropic stochastic electrostatic potential is considered from a semi-analytic point of view. The analysis is performed in the weak turbulence limit and as an analytical tool the decorrelation trajectory method is used. It is shown that the fragmentation of the drift wave structures (a signature of the zonal flow generation) is influenced not only by the anisotropy parameter and the electrostatic Kubo number as expected, but also by the diamagnetic Kubo number. Global Lagrangian averages of characteristic quantities are calculated and interpreted

  10. Zonal flows and turbulence in fluids and plasmas

    Science.gov (United States)

    Parker, Jeffrey Bok-Cheung

    In geophysical and plasma contexts, zonal flows are well known to arise out of turbulence. We elucidate the transition from statistically homogeneous turbulence without zonal flows to statistically inhomogeneous turbulence with steady zonal flows. Starting from the Hasegawa--Mima equation, we employ both the quasilinear approximation and a statistical average, which retains a great deal of the qualitative behavior of the full system. Within the resulting framework known as CE2, we extend recent understanding of the symmetry-breaking 'zonostrophic instability'. Zonostrophic instability can be understood in a very general way as the instability of some turbulent background spectrum to a zonally symmetric coherent mode. As a special case, the background spectrum can consist of only a single mode. We find that in this case the dispersion relation of zonostrophic instability from the CE2 formalism reduces exactly to that of the 4-mode truncation of generalized modulational instability. We then show that zonal flows constitute pattern formation amid a turbulent bath. Zonostrophic instability is an example of a Type I s instability of pattern-forming systems. The broken symmetry is statistical homogeneity. Near the bifurcation point, the slow dynamics of CE2 are governed by a well-known amplitude equation, the real Ginzburg-Landau equation. The important features of this amplitude equation, and therefore of the CE2 system, are multiple. First, the zonal flow wavelength is not unique. In an idealized, infinite system, there is a continuous band of zonal flow wavelengths that allow a nonlinear equilibrium. Second, of these wavelengths, only those within a smaller subband are stable. Unstable wavelengths must evolve to reach a stable wavelength; this process manifests as merging jets. These behaviors are shown numerically to hold in the CE2 system, and we calculate a stability diagram. The stability diagram is in agreement with direct numerical simulations of the quasilinear

  11. Statistics of lower tropospheric inversions over the continental United States

    Energy Technology Data Exchange (ETDEWEB)

    Zhang, Y.H.; Zhang, S.D.; Yi, F. [Wuhan Univ., Hubei (China). School of Electronic Information; Ministry of Education, Wuhan, Hubei (China). Key Lab. of Geospace Environment and Geodesy; State Observatory for Atmospheric Remote Sensing, Wuhan (China); Chen, Z.Y. [Chinese Academy of Sciences, Beijing (China). Inst. of Atmospheric Sciences

    2011-07-01

    The basic structure parameters of lower tropospheric inversions (LTIs) have been derived from 10 years (1998-2007) of high vertical resolution ({proportional_to}50 m) radiosonde observations over 56 United States stations. Seasonal and longitudinal variability of these parameters are presented and the formation mechanisms of LTI are also discussed. It is found that LTI seems to be a common feature over the continental United States. The LTI occurrence rates (defined as the fraction of measurements with LTI, which is calculated from the number of LTI cases divided by the number of measurements of the whole 10 years) at these 56 stations vary from 3.7% to 14.5%; the averaged base heights of LTI have a range of 3-5 km above mean sea level (a.m.s.l.); the averaged thicknesses and temperature jump ranges from 420-465m and 1.9-2.2 K, respectively. These parameters have an obvious seasonal variation. In winter, all the occurrence rates, thicknesses and temperature jumps of LTI have much larger values than those in summer. LTI occurrence rate shows an obvious west-east increasing trend in all 4 seasons. Detailed analyses reveal that dynamical instability induced by strong zonal wind shear is responsible for LTI in winter, spring and autumn; the frontal system tends to generate LTI in summer. Since the higher occurrence rate, larger temperature jump and larger thickness of LTI occur in winter, we believe strong zonal wind shear plays a more important role in the formation of LTI. (orig.)

  12. Statistics of lower tropospheric inversions over the continental United States

    Directory of Open Access Journals (Sweden)

    Y. H. Zhang

    2011-02-01

    Full Text Available The basic structure parameters of lower tropospheric inversions (LTIs have been derived from 10 years (1998–2007 of high vertical resolution (~50 m radiosonde observations over 56 United States stations. Seasonal and longitudinal variability of these parameters are presented and the formation mechanisms of LTI are also discussed. It is found that LTI seems to be a common feature over the continental United States. The LTI occurrence rates (defined as the fraction of measurements with LTI, which is calculated from the number of LTI cases divided by the number of measurements of the whole 10 years at these 56 stations vary from 3.7% to 14.5%; the averaged base heights of LTI have a range of 3–5 km above mean sea level (a.m.s.l.; the averaged thicknesses and temperature jump ranges from 420–465 m and 1.9–2.2 K, respectively. These parameters have an obvious seasonal variation. In winter, all the occurrence rates, thicknesses and temperature jumps of LTI have much larger values than those in summer. LTI occurrence rate shows an obvious west-east increasing trend in all 4 seasons. Detailed analyses reveal that dynamical instability induced by strong zonal wind shear is responsible for LTI in winter, spring and autumn; the frontal system tends to generate LTI in summer. Since the higher occurrence rate, larger temperature jump and larger thickness of LTI occur in winter, we believe strong zonal wind shear plays a more important role in the formation of LTI.

  13. Zonal asymmetry of daytime 150-km echoes observed by Equatorial Atmosphere Radar in Indonesia

    Directory of Open Access Journals (Sweden)

    T. Yokoyama

    2009-03-01

    Full Text Available Multi-beam observations of the daytime ionospheric E-region irregularities and the so-called 150-km echoes with the 47-MHz Equatorial Atmosphere Radar (EAR in West Sumatra, Indonesia (0.20° S, 100.32° E, 10.36° S dip latitude are presented. 150-km echoes have been frequently observed by the EAR, and their characteristics are basically the same as the equatorial ones, except for an intriguing zonal asymmetry; stronger echoes in lower altitudes in the east directions, and weaker echoes in higher altitudes in the west. The highest occurrence is seen at 5.7° east with respect to the magnetic meridian, and the altitude gradually increases as viewing from the east to west. Arc structures which return backscatter echoes are proposed to explain the asymmetry. While the strength of radar echoes below 105 km is uniform within the wide coverage of azimuthal directions, the upper E-region (105–120 km echoes also show a different type of zonal asymmetry, which should be generated by an essentially different mechanism from the lower E-region and 150-km echoes.

  14. Parasitic Diseases of Ruminants Brought to Two Zonal Veterinary ...

    African Journals Online (AJOL)

    A five years study (2003-2007) of parasitic diseases of ruminants brought to two Zonal Veterinary clinics located in the Southern part of Niger State, Central Nigeria was carried out to establish disease patterns in cattle, sheep and goats. The study was based on the data extracted from the monthly records of parasitic disease ...

  15. Improvement of OMI Ozone Profile Retrievals in the Troposphere and Lower Troposphere by the Use of the Tropopause-Based Ozone Profile Climatology

    Science.gov (United States)

    Bak, Juseon; Liu, X.; Wei, J.; Kim, J. H.; Chance, K.; Barnet, C.

    2011-01-01

    An advance algorithm based on the optimal estimation technique has beeen developed to derive ozone profile from GOME UV radiances and have adapted it to OMI UV radiances. OMI vertical resolution : 7-11 km in the troposphere and 10-14 km in the stratosphere. Satellite ultraviolet measurements (GOME, OMI) contain little vertical information for the small scale of ozone, especially in the upper troposphere (UT) and lower stratosphere (LS) where the sharp O3 gradient across the tropopause and large ozone variability are observed. Therefore, retrievals depend greatly on the a-priori knowledge in the UTLS

  16. Forecasting tropical cyclone recurvature with upper tropospheric winds

    Science.gov (United States)

    Gentry, R. C.

    1983-01-01

    Data from 17 tropical cyclones during the 1974 through 1979 hurricane seasons are used to investigate whether the high level winds far to the northwest, north and northeast of the hurricane center can be used to predict hurricane track recurvature. When the man 200-mb winds 1500 to 2000 km northwest and north of the storm center equal or exceed 20 m/s, 80 per cent of the storms recurved before traveling as much as 12 degrees of longitude farther west. The high winds were also used to predict change in direction of forward motion during the next 72 hours. The regression equations developed explain up to 41 per cent of the variance in future direction. In addition to the geostrophic winds used, winds were also obtained by tracking clouds with successive satellite imagery. The u-components of the satellite winds are highly correlated with the geostrophic winds at 200-mb and could probably be used instead of them when available. The v-components are less highly correlated.

  17. Interannual variations in the zonal asymmetry of the subpolar latitudes total ozone column during the austral spring

    Directory of Open Access Journals (Sweden)

    Eduardo A. Agosta

    2010-06-01

    Full Text Available The Southern Hemisphere midlatitude Total Ozone Column (TOC shows a horseshoe like structure with a minimum which appears to have two preferential extreme positions during October: one, near southern South America, the other, near the Greenwich Meridian approximately. The interannual zonal ozone asymmetry exists independently of the variations induced by the 11-year solar cycle, the Quasi-Biennial Oscillation (QBO and planetary wave activity inducing the Brewer-Dobson circulation. The classification and climatological composition of these two extreme ozone-minimum positions allows for the observations of statistically significant patterns in geopotential height and zonal winds associated with the quasi-stationary wave 1, extending throughout lower stratosphere. The changes in the quasi-stationary wave 1 associated with the extreme TOC positions appear to have sinks and sources determining transient interactions between troposphere and the stratosphere. Thus, distinct climate states in the troposphere seem to be dynamically linked with the state of the stratosphere and ozone layer. The migration of the TOC trough from southern South America to the east during the 1990s can be related to changes in the troposphere/stratosphere coupling through changes in the Southern Annular Mode variability in spring.La Columna Total de Ozono (CTO de las latitudes medias del Hemisferio Sur muestra una estructura de herradura con un mínimo que muestra tener dos posiciones preferenciales extremas durante octubre: uno, en las cercanías del sur de Sudamérica, y el otro, cerca del meridiano de Greenwich. La asimetría zonal de ozono existe independientemente de las variaciones inducidas por el ciclo solar de 11 años, la Oscilación Cuasi-Bianual (QBO y la actividad de onda planetaria asociada a la circulación de Brewer-Dobson. La clasificación y composición climatológica de estas dos situaciones longitudinalmente extremas de mínimo de ozono permite observar

  18. How does Interactive Chemistry Influence the Representation of Stratosphere-Troposphere Coupling in a Climate Model?

    Science.gov (United States)

    Haase, S.; Matthes, K. B.

    2017-12-01

    Changes in stratospheric ozone can trigger tropospheric circulation changes. In the Southern hemisphere (SH), the observed shift of the Southern Annular Mode was attributed to the observed trend in lower stratospheric ozone. In the Northern Hemisphere (NH), a recent study showed that extremely low stratospheric ozone conditions during spring produce robust anomalies in the troposphere (zonal wind, temperature and precipitation). This could only be reproduced in a coupled chemistry climate model indicating that chemical-dynamical feedbacks are also important on the NH. To further investigate the importance of interactive chemistry for surface climate, we conducted a set of experiments using NCAR's Community Earth System Model (CESM1) with the Whole Atmosphere Community Climate Model (WACCM) as the atmosphere component. WACCM contains a fully interactive stratospheric chemistry module in its standard configuration. It also allows for an alternative configuration, referred to as SC-WACCM, in which the chemistry (O3, NO, O, O2, CO2 and chemical and shortwave heating rates) is specified as a 2D field in the radiation code. A comparison of the interactive vs. the specified chemistry version enables us to evaluate the relative importance of interactive chemistry by systematically inhibiting the feedbacks between chemistry and dynamics. To diminish the effect of temporal interpolation when prescribing ozone, we use daily resolved zonal mean ozone fields for the specified chemistry run. Here, we investigate the differences in stratosphere-troposphere coupling between the interactive and specified chemistry simulations for the mainly chemically driven SH as well as for the mainly dynamically driven NH. We will especially consider years that are characterized by extremely low stratospheric ozone on the one hand and by large dynamical disturbances, i.e. Sudden Stratospheric Warmings, on the other hand.

  19. Representativeness of single lidar stations for zonally averaged ozone profiles, their trends and attribution to proxies

    Directory of Open Access Journals (Sweden)

    C. Zerefos

    2018-05-01

    Full Text Available This paper is focusing on the representativeness of single lidar stations for zonally averaged ozone profile variations over the middle and upper stratosphere. From the lower to the upper stratosphere, ozone profiles from single or grouped lidar stations correlate well with zonal means calculated from the Solar Backscatter Ultraviolet Radiometer (SBUV satellite overpasses. The best representativeness with significant correlation coefficients is found within ±15° of latitude circles north or south of any lidar station. This paper also includes a multivariate linear regression (MLR analysis on the relative importance of proxy time series for explaining variations in the vertical ozone profiles. Studied proxies represent variability due to influences outside of the earth system (solar cycle and within the earth system, i.e. dynamic processes (the Quasi Biennial Oscillation, QBO; the Arctic Oscillation, AO; the Antarctic Oscillation, AAO; the El Niño Southern Oscillation, ENSO, those due to volcanic aerosol (aerosol optical depth, AOD, tropopause height changes (including global warming and those influences due to anthropogenic contributions to atmospheric chemistry (equivalent effective stratospheric chlorine, EESC. Ozone trends are estimated, with and without removal of proxies, from the total available 1980 to 2015 SBUV record. Except for the chemistry related proxy (EESC and its orthogonal function, the removal of the other proxies does not alter the significance of the estimated long-term trends. At heights above 15 hPa an inflection point between 1997 and 1999 marks the end of significant negative ozone trends, followed by a recent period between 1998 and 2015 with positive ozone trends. At heights between 15 and 40 hPa the pre-1998 negative ozone trends tend to become less significant as we move towards 2015, below which the lower stratosphere ozone decline continues in agreement with findings of recent literature.

  20. Representativeness of single lidar stations for zonally averaged ozone profiles, their trends and attribution to proxies

    Science.gov (United States)

    Zerefos, Christos; Kapsomenakis, John; Eleftheratos, Kostas; Tourpali, Kleareti; Petropavlovskikh, Irina; Hubert, Daan; Godin-Beekmann, Sophie; Steinbrecht, Wolfgang; Frith, Stacey; Sofieva, Viktoria; Hassler, Birgit

    2018-05-01

    This paper is focusing on the representativeness of single lidar stations for zonally averaged ozone profile variations over the middle and upper stratosphere. From the lower to the upper stratosphere, ozone profiles from single or grouped lidar stations correlate well with zonal means calculated from the Solar Backscatter Ultraviolet Radiometer (SBUV) satellite overpasses. The best representativeness with significant correlation coefficients is found within ±15° of latitude circles north or south of any lidar station. This paper also includes a multivariate linear regression (MLR) analysis on the relative importance of proxy time series for explaining variations in the vertical ozone profiles. Studied proxies represent variability due to influences outside of the earth system (solar cycle) and within the earth system, i.e. dynamic processes (the Quasi Biennial Oscillation, QBO; the Arctic Oscillation, AO; the Antarctic Oscillation, AAO; the El Niño Southern Oscillation, ENSO), those due to volcanic aerosol (aerosol optical depth, AOD), tropopause height changes (including global warming) and those influences due to anthropogenic contributions to atmospheric chemistry (equivalent effective stratospheric chlorine, EESC). Ozone trends are estimated, with and without removal of proxies, from the total available 1980 to 2015 SBUV record. Except for the chemistry related proxy (EESC) and its orthogonal function, the removal of the other proxies does not alter the significance of the estimated long-term trends. At heights above 15 hPa an inflection point between 1997 and 1999 marks the end of significant negative ozone trends, followed by a recent period between 1998 and 2015 with positive ozone trends. At heights between 15 and 40 hPa the pre-1998 negative ozone trends tend to become less significant as we move towards 2015, below which the lower stratosphere ozone decline continues in agreement with findings of recent literature.

  1. Tropospheric ozone climatology at two Southern Hemisphere tropical/subtropical sites, (Reunion Island and Irene, South Africa from ozonesondes, LIDAR, and in situ aircraft measurements

    Directory of Open Access Journals (Sweden)

    G. Clain

    2009-03-01

    Full Text Available This paper presents a climatology and trends of tropospheric ozone in the Southwestern Indian Ocean (Reunion Island and South Africa (Irene and Johannesburg. This study is based on a multi-instrumental dataset: PTU-O3 ozonesondes, DIAL LIDAR and MOZAIC airborne instrumentation.

    The seasonal profiles of tropospheric ozone at Reunion Island have been calculated from two different data sets: ozonesondes and LIDAR. The two climatological profiles are similar, except in austral summer when the LIDAR profiles show greater values in the free troposphere, and in the upper troposphere when the LIDAR profiles show lower values during all seasons. These results show that the climatological value of LIDAR profiles must be discussed with care since LIDAR measurements can be performed only under clear sky conditions, and the upper limit of the profile depends on the signal strength.

    In addition, linear trends have been calculated from ozonesonde data at Reunion and Irene. Considering the whole tropospheric column, the trend is slightly positive for Reunion, and more clearly positive for Irene. Trend calculations have also been made separating the troposphere into three layers, and separating the dataset into seasons. Results show that the positive trend for Irene is governed by the lower layer that is affected by industrial pollution and biomass burning. On the contrary, for Reunion Island, the strongest trends are observed in the upper troposphere, and in winter when stratosphere-troposphere exchange is more frequently expected.

  2. Evidence of a tropospheric aerosol backscatter background mode

    Science.gov (United States)

    Rothermel, Jeffry; Bowdle, David A.; Vaughan, J. Michael; Post, Madison J.

    1989-01-01

    Vertical profiles of atmospheric aerosol backscatter coefficients at 10.6 microns obtained with airborne and ground-based lidar are compared. Both sets of profiles show a high frequency of occurrence of low backscatter over a limited range of values in the middle and upper troposphere. It is suggested that this narrow range indicates a ubiquitous background mode for atmospheric backscatter around the globe. Implications of such a mode for global scale aerosol models and for the design of satellite-borne lidar-based sensors are discussed.

  3. Tropospheric aerosol backscatter background mode at CO2 wavelengths

    Science.gov (United States)

    Rothermel, Jeffry; Bowdle, David A.; Menzies, Robert T.; Post, Madison J.; Vaughan, J. Michael

    1989-01-01

    A comparison is made between three climatologies of backscatter measurements in the troposphere and lower stratosphere at CO2 wavelengths. These were obtained from several locations using ground-based and airborne lidar systems. All three measurement sets show similar features, specifically, a high frequency of occurrence of low backscatter over a limited range of values in the middle and upper atmosphere (the 'background mode'). This background mode is important for the design and performance simulation of the prospective satellite sensors that rely on atmospheric aerosols as scattering targets.

  4. Treatment of dynamical processes in two-dimensional models of the troposphere and stratosphere

    International Nuclear Information System (INIS)

    Wuebbles, D.J.

    1980-07-01

    The physical structure of the troposphere and stratosphere is the result of an intricate interplay among a large number of radiative, chemical, and dynamical processes. Because it is not possible to model the global environment in the laboratory, theoretical models must be relied on, subject to observational verification, to simulate atmospheric processes. Of particular concern in recent years has been the modeling of those processes affecting the structure of ozone and other trace species in the stratosphere and troposphere. Zonally averaged two-dimensional models with spatial resolution in the vertical and meridional directions can provide a much more realistic representation of tracer transport than one-dimensional models, yet are capable of the detailed representation of chemical and radiative processes contained in the one-dimensional models. The purpose of this study is to describe and analyze existing approaches to representing global atmospheric transport processes in two-dimensional models and to discuss possible alternatives to these approaches. A general description of the processes controlling the transport of trace constituents in the troposphere and stratosphere is given

  5. Evidence of Convective Redistribution of Carbon Monoxide in Aura Tropospheric Emission Sounder (TES) and Microwave Limb Sounder (MLS) Observations

    Science.gov (United States)

    Manyin, Michael; Douglass, Anne; Schoeberl, Mark

    2010-01-01

    Vertical convective transport is a key element of the tropospheric circulation. Convection lofts air from the boundary layer into the free troposphere, allowing surface emissions to travel much further, and altering the rate of chemical processes such as ozone production. This study uses satellite observations to focus on the convective transport of CO from the boundary layer to the mid and upper troposphere. Our hypothesis is that strong convection associated with high rain rate regions leads to a correlation between mid level and upper level CO amounts. We first test this hypothesis using the Global Modeling Initiative (GMI) chemistry and transport model. We find the correlation is robust and increases as the precipitation rate (the strength of convection) increases. We next examine three years of CO profiles from the Tropospheric Emission Sounder (TES) and Microwave Limb Sounder (MLS) instruments aboard EOS Aura. Rain rates are taken from the Tropical Rainfall Measuring Mission (TRMM) 3B-42 multi-satellite product. Again we find a correlation between mid-level and upper tropospheric CO, which increases with rain rate. Our result shows the critical importance of tropical convection in coupling vertical levels of the troposphere in the transport of trace gases. The effect is seen most clearly in strong convective regions such as the Inter-tropical Convergence Zone.

  6. Aerosol indirect effect on tropospheric ozone via lightning

    Science.gov (United States)

    Yuan, T.; Remer, L. A.; Bian, H.; Ziemke, J. R.; Albrecht, R. I.; Pickering, K. E.; Oreopoulos, L.; Goodman, S. J.; Yu, H.; Allen, D. J.

    2012-12-01

    Tropospheric ozone (O3) is a pollutant and major greenhouse gas and its radiative forcing is still uncertain. The unresolved difference between modeled and observed natural background O3 concentrations is a key source of the uncertainty. Here we demonstrate remarkable sensitivity of lightning activity to aerosol loading with lightning activity increasing more than 30 times per unit of aerosol optical depth over our study area. We provide observational evidence that indicates the observed increase in lightning activity is caused by the influx of aerosols from a volcano. Satellite data analyses suggest O3 is increased as a result of aerosol-induced increase in lightning and lightning produced NOx. Model simulations with prescribed lightning change corroborate the satellite data analysis. This aerosol-O3 connection is achieved via aerosol increasing lightning and thus lightning produced nitrogen oxides. This aerosol-lightning-ozone link provides a potential physical mechanism that may account for a part of the model-observation difference in background O3 concentration. More importantly, O3 production increase from this link is concentrated in the upper troposphere, where O3 is most efficient as a greenhouse gas. Both of these implications suggest a stronger O3 historical radiative forcing. This introduces a new pathway, through which increasing in aerosols from pre-industrial time to present day enhances tropospheric O3 production. Aerosol forcing thus has a warming component via its effect on O3 production. Sensitivity simulations suggest that 4-8% increase of tropospheric ozone, mainly in the tropics, is expected if aerosol-lighting-ozone link is parameterized, depending on the background emission scenario. We note, however, substantial uncertainties remain on the exact magnitude of aerosol effect on tropospheric O3 via lightning. The challenges for obtaining a quantitative global estimate of this effect are also discussed. Our results have significant implications

  7. Instrumentation for tropospheric aerosol characterization

    Energy Technology Data Exchange (ETDEWEB)

    Shi, Z.; Young, S.E.; Becker, C.H.; Coggiola, M.J. [SRI International, Menlo Park, CA (United States); Wollnik, H. [Giessen Univ. (Germany)

    1997-12-31

    A new instrument has been developed that determines the abundance, size distribution, and chemical composition of tropospheric and lower stratospheric aerosols with diameters down to 0.2 {mu}m. In addition to aerosol characterization, the instrument also monitors the chemical composition of the ambient gas. More than 25.000 aerosol particle mass spectra were recorded during the NASA-sponsored Subsonic Aircraft: Contrail and Cloud Effects Special Study (SUCCESS) field program using NASA`s DC-8 research aircraft. (author) 7 refs.

  8. Instrumentation for tropospheric aerosol characterization

    Energy Technology Data Exchange (ETDEWEB)

    Shi, Z; Young, S E; Becker, C H; Coggiola, M J [SRI International, Menlo Park, CA (United States); Wollnik, H [Giessen Univ. (Germany)

    1998-12-31

    A new instrument has been developed that determines the abundance, size distribution, and chemical composition of tropospheric and lower stratospheric aerosols with diameters down to 0.2 {mu}m. In addition to aerosol characterization, the instrument also monitors the chemical composition of the ambient gas. More than 25.000 aerosol particle mass spectra were recorded during the NASA-sponsored Subsonic Aircraft: Contrail and Cloud Effects Special Study (SUCCESS) field program using NASA`s DC-8 research aircraft. (author) 7 refs.

  9. Analysis of the summertime buildup of tropospheric ozone abundances over the Middle East and North Africa as observed by the Tropospheric Emission Spectrometer instrument

    Science.gov (United States)

    Liu, Jane J.; Jones, Dylan B. A.; Worden, John R.; Noone, David; Parrington, Mark; Kar, Jay

    2009-03-01

    We use the GEOS-Chem chemical transport model to interpret observations of tropospheric ozone from the Tropospheric Emission Spectrometer (TES) satellite instrument in summer 2005. Observations from TES reveal elevated ozone in the middle troposphere (500-400 hPa) across North Africa and the Middle East. Observed ozone abundances in the middle troposphere are at a maximum in summer and a minimum in winter, consistent with the previously predicted summertime "Middle East ozone maximum." This summertime enhancement in ozone is associated with the Arabian and Sahara anticyclones, centered over the Zagros and Atlas Mountains, respectively. These anticyclones isolate the middle troposphere over northeast Africa and the Middle East, with westerlies to the north and easterlies to the south, facilitating the buildup of ozone. Over the Middle East, we find that in situ production and transport from Asia provides comparable contributions of 30-35% to the ozone buildup. Over North Africa, in situ production is dominant (at about 20%), with transport from Asia, North America, and equatorial Africa each contributing about 10-15% to the total ozone. We find that although the eastern Mediterranean is characterized by strong descent in the middle and upper troposphere in summer, transport from the boundary layer accounts for about 25% of the local Middle Eastern contribution to the ozone enhancement in the middle troposphere. This upward transport of boundary layer air is associated with orographic lifting along the Zagros Mountains in Iran and the Asir and Hijaz Mountain ranges in Saudi Arabia, and is consistent with TES observations of deuterated water.

  10. The global warming potential of methane reassessed with combined stratosphere and troposphere chemistry

    Science.gov (United States)

    Holmes, C. D.; Archibald, A. T.; Eastham, S. D.; Søvde, O. A.

    2017-12-01

    Methane is a direct and indirect greenhouse gas. The direct greenhouse effect comes from the radiation absorbed and emitted by methane itself. The indirect greenhouse effect comes from radiatively active gases that are produced during methane oxidation: principally O3, H2O, and CO2. Methane also suppresses tropospheric OH, which indirectly affects numerous greenhouses gases and aerosols. Traditionally, the methane global warming potential (GWP) has included the indirect effects on tropospheric O3 and OH and stratospheric H2O, with these effects estimated independently from unrelated tropospheric and stratospheric chemistry models and observations. Using this approach the CH4 is about 28 over 100 yr (without carbon cycle feedbacks, IPCC, 2013). Here we present a comprehensive analysis of the CH4 GWP in several 3-D global atmospheric models capable of simulating both tropospheric and stratospheric chemistry (GEOS-Chem, Oslo CTM3, UKCA). This enables us to include, for the first time, the indirect effects of CH4 on stratospheric O3 and stratosphere-troposphere coupling. We diagnose the GWP from paired simulations with and without a 5% perturbation to tropospheric CH4 concentrations. Including stratospheric chemistry nearly doubles the O3 contribution to CH4 GWP because of O3 production in the lower stratosphere and because CH4 inhibits Cl-catalyzed O3 loss in the upper stratosphere. In addition, stratosphere-troposphere coupling strengthens the chemical feedback on its own lifetime. In the stratosphere, this feedback operates by a CH4 perturbation thickening the stratospheric O3 layer, which impedes UV-driven OH production in the troposphere and prolongs the CH4 lifetime. We also quantify the impact of CH4-derived H2O on the stratospheric HOx cycles but these effects are small. Combining all of the above, these models suggest that the 100-yr GWP of CH4 is over 33.5, a 20% increase over the latest IPCC assessment.

  11. Cost-Optimal ATCs in Zonal Electricity Markets

    DEFF Research Database (Denmark)

    Jensen, Tue Vissing; Kazempour, Jalal; Pinson, Pierre

    2017-01-01

    from the physical ATCs based on security indices only typically used in zonal electricity markets today. Determining cost-optimal ATCs requires viewing ATCs as an endogenous market construct, and leads naturally to the definition of a market entity whose responsibility is to optimize ATCs....... The optimization problem which this entity solves is a stochastic bilevel problem, which we decompose to yield a computationally tractable formulation. We show that cost-optimal ATCs depend non-trivially on the underlying network structure, and the problem of finding a setof cost-optimal ATCs is in general non...... by a factor of 2 or more, and ATCs which are zero between well-connected areas.Our results indicate that the perceived efficiency gap between zonal and nodal markets may be exagerrated if non-optimal ATCs are used....

  12. Diffusion of Zonal Variables Using Node-Centered Diffusion Solver

    Energy Technology Data Exchange (ETDEWEB)

    Yang, T B

    2007-08-06

    Tom Kaiser [1] has done some preliminary work to use the node-centered diffusion solver (originally developed by T. Palmer [2]) in Kull for diffusion of zonal variables such as electron temperature. To avoid numerical diffusion, Tom used a scheme developed by Shestakov et al. [3] and found their scheme could, in the vicinity of steep gradients, decouple nearest-neighbor zonal sub-meshes leading to 'alternating-zone' (red-black mode) errors. Tom extended their scheme to couple the sub-meshes with appropriate chosen artificial diffusion and thereby solved the 'alternating-zone' problem. Because the choice of the artificial diffusion coefficient could be very delicate, it is desirable to use a scheme that does not require the artificial diffusion but still able to avoid both numerical diffusion and the 'alternating-zone' problem. In this document we present such a scheme.

  13. Zonally averaged chemical-dynamical model of the lower thermosphere

    International Nuclear Information System (INIS)

    Kasting, J.F.; Roble, R.G.

    1981-01-01

    A zonally averaged numerical model of the thermosphere is used to examine the coupling between neutral composition, including N 2 , O 2 and O, temperature, and winds at solstice for solar minimum conditions. The meridional circulation forced by solar heating results in a summer-to-winter flow, with a winter enhancement in atomic oxygen density that is a factor of about 1.8 greater than the summer hemisphere at 160 km. The O 2 and N 2 variations are associated with a latitudinal gradient in total number density, which is required to achieve pressure balance in the presence of large zonal jets. Latitudinal profiles OI (5577A) green line emission intensity are calculated by using both Chapman and Barth mechanisms. Composition of the lower thermosphere is shown to be strongly influenced by circulation patterns initiated in the stratosphere and lower mesosphere, below the lower boundary used in the model

  14. Statistical properties of Charney-Hasegawa-Mima zonal flows

    International Nuclear Information System (INIS)

    Anderson, Johan; Botha, G. J. J.

    2015-01-01

    A theoretical interpretation of numerically generated probability density functions (PDFs) of intermittent plasma transport events in unforced zonal flows is provided within the Charney-Hasegawa-Mima (CHM) model. The governing equation is solved numerically with various prescribed density gradients that are designed to produce different configurations of parallel and anti-parallel streams. Long-lasting vortices form whose flow is governed by the zonal streams. It is found that the numerically generated PDFs can be matched with analytical predictions of PDFs based on the instanton method by removing the autocorrelations from the time series. In many instances, the statistics generated by the CHM dynamics relaxes to Gaussian distributions for both the electrostatic and vorticity perturbations, whereas in areas with strong nonlinear interactions it is found that the PDFs are exponentially distributed

  15. Secondary ozone peaks in the troposphere over the Himalayas

    Directory of Open Access Journals (Sweden)

    N. Ojha

    2017-06-01

    Full Text Available Layers with strongly enhanced ozone concentrations in the middle–upper troposphere, referred to as secondary ozone peaks (SOPs, have been observed in different regions of the world. Here we use the global ECHAM5/MESSy atmospheric chemistry model (EMAC to (i investigate the processes causing SOPs, (ii explore both their frequency of occurrence and seasonality, and (iii assess their effects on the tropospheric ozone budget over the Himalayas. The vertical profiles of potential vorticity (PV and a stratospheric ozone tracer (O3s in EMAC simulations, in conjunction with the structure of SOPs, suggest that SOPs over the Himalayas are formed by stratosphere-to-troposphere transport (STT of ozone. The spatial distribution of O3s further shows that such effects are in general most pronounced in the northern part of India. Model simulated ozone distributions and backward air trajectories show that ozone rich air masses, associated with STT, originate as far as northern Africa and the North Atlantic Ocean, the Middle East, as well as in nearby regions in Afghanistan and Pakistan, and are rapidly (within 2–3 days transported to the Himalayas. Analysis of a 15-year (2000–2014 EMAC simulation shows that the frequency of SOPs is highest during the pre-monsoon season (e.g. 11 % of the time in May, while no intense SOP events are found during the July–October period. The SOPs are estimated to enhance the tropospheric column ozone (TCO over the central Himalayas by up to 21 %.

  16. Variations of tropospheric methane over Japan during 1988–2010

    Directory of Open Access Journals (Sweden)

    Taku Umezawa

    2014-05-01

    Full Text Available We present observations of CH4 concentrations from the lower to upper troposphere (LT and UT over Japan during 1988–2010 based on aircraft measurements from the Tohoku University (TU. The analysis is aided by simulation results using an atmospheric chemistry transport model (i.e. ACTM. Tropospheric CH4 over Japan shows interannual and seasonal variations that are dependent on altitudes, primarily reflecting differences in air mass origins at different altitudes. The long-term trend and interannual variation of CH4 in the LT are consistent with previous reports of measurements at surface baseline stations in the northern hemisphere. However, those in the UT show slightly different features from those in the LT. In the UT, CH4 concentrations show a seasonal maximum in August due to efficient transport of air masses influenced by continental CH4 sources, while LT CH4 reaches its seasonal minimum during summer due to enhanced chemical loss. Vertical profiles of the CH4 concentrations also vary with season, reflecting the seasonal cycles at the respective altitudes. In summer, transport of CH4-rich air from Asian regions elevates UT CH4 levels, forming a uniform vertical profile above the mid-troposphere. On the other hand, CH4 decreases nearly monotonically with altitude in winter–spring. The ACTM simulations with different emission scenarios reproduce general features of the tropospheric CH4 variations over Japan. Tagged tracer simulations using the ACTM indicate substantial contributions of CH4 sources in South Asia and East Asia to the summertime high CH4 values observed in the UT. This suggests that our observations over Japan are highly sensitive to CH4 emission signals particularly from Asia.

  17. Zonal flow dynamics and control of turbulent transport in stellarators.

    Science.gov (United States)

    Xanthopoulos, P; Mischchenko, A; Helander, P; Sugama, H; Watanabe, T-H

    2011-12-09

    The relation between magnetic geometry and the level of ion-temperature-gradient (ITG) driven turbulence in stellarators is explored through gyrokinetic theory and direct linear and nonlinear simulations. It is found that the ITG radial heat flux is sensitive to details of the magnetic configuration that can be understood in terms of the linear behavior of zonal flows. The results throw light on the question of how the optimization of neoclassical confinement is related to the reduction of turbulence.

  18. Global characteristics of zonal flows generated by ion temperature gradient driven turbulence in tokamak plasmas

    International Nuclear Information System (INIS)

    Miyato, Naoaki; Kishimoto, Yasuaki; Li, Jiquan

    2004-08-01

    Global structure of zonal flows driven by ion temperature gradient driven turbulence in tokamak plasmas is investigated using a global electromagnetic Landau fluid code. Characteristics of the coupled system of the zonal flows and the turbulence change with the safety factor q. In a low q region stationary zonal flows are excited and suppress the turbulence effectively. Coupling between zonal flows and poloidally asymmetric pressure perturbations via a geodesic curvature makes the zonal flows oscillatory in a high q region. Also we identify energy transfer from the zonal flows to the turbulence via the poloidally asymmetric pressure perturbations in the high q region. Therefore in the high q region the zonal flows cannot quench the turbulent transport completely. (author)

  19. The relevance of grid expansion under zonal markets

    International Nuclear Information System (INIS)

    Bertsch, Joachim; Hagspiel, Simeon; Just, Lisa

    2015-01-01

    The European electricity market design is based on zonal markets with uniform prices. Locational price signals within these zones - necessary to ensure long-term efficiency - are not provided. Specifically, if intra-zonal congestion occurs due to missing grid expansion, the market design is revealed as inherently incomplete. This might lead to severe, unwanted distortions of the electricity market, both in the short- and in the long-term. In this paper, we study these distortions with a specific focus on the impact of restricted grid expansion under zonal markets. For this, we use a long term fundamental dispatch and investment model of the European electricity system and gradually restrict the allowed expansion of the transmission grid per decade. We find that the combination of an incomplete market design and restricted grid expansion leads to a misallocation of generation capacities and the inability to transport electricity to where it is needed. Consequences are severe and lead to load curtailment of up to 2-3 %. Moreover, missing grid expansion makes it difficult and costly to reach envisaged energy targets in the power sector. Hence, we argue that in the likely event of restricted grid expansion, either administrative measures or - presumably more efficient - an adaptation of the current market design to include locational signals will become necessary.

  20. The relevance of grid expansion under zonal markets

    Energy Technology Data Exchange (ETDEWEB)

    Bertsch, Joachim; Hagspiel, Simeon; Just, Lisa [ewi Energy Research and Scenarios gGmbH, Cologne (Germany); Cologne Univ. (Germany). Dept. of Economics; Brown, Tom [Frankfurt Institute of Advanced Studies (Germany)

    2015-12-15

    The European electricity market design is based on zonal markets with uniform prices. Locational price signals within these zones - necessary to ensure long-term efficiency - are not provided. Specifically, if intra-zonal congestion occurs due to missing grid expansion, the market design is revealed as inherently incomplete. This might lead to severe, unwanted distortions of the electricity market, both in the short- and in the long-term. In this paper, we study these distortions with a specific focus on the impact of restricted grid expansion under zonal markets. For this, we use a long term fundamental dispatch and investment model of the European electricity system and gradually restrict the allowed expansion of the transmission grid per decade. We find that the combination of an incomplete market design and restricted grid expansion leads to a misallocation of generation capacities and the inability to transport electricity to where it is needed. Consequences are severe and lead to load curtailment of up to 2-3 %. Moreover, missing grid expansion makes it difficult and costly to reach envisaged energy targets in the power sector. Hence, we argue that in the likely event of restricted grid expansion, either administrative measures or - presumably more efficient - an adaptation of the current market design to include locational signals will become necessary.

  1. Tropospheric effects of energy conversion

    International Nuclear Information System (INIS)

    Derwent, R.G.

    1992-01-01

    The tropospheric concentrations of a number of trace gases are increasing due to man's activities. For some trace gases, their atmospheric life cycles are not fully understood and it is difficult to be certain about the role of man's activities. Emissions from the energy industries and energy conversion processes represent an important subset of source terms in these life cycles, along with agriculture, deforestation, cement manufacture, biomass burning, process industries and natural biospheric processes. Global Warming Potentials (GWPs) allow the tropospheric effects of a range of climate forcing trace gases to be assessed on a comparable basis. If a short term view of the commitment to global warming is adopted then the contribution from other trace gases may approach and exceed that of carbon dioxide, itself. Over longer time horizons, the long atmospheric lifetime of carbon dioxide shows through as a major influence and the contributions from the other trace gases appear to be much smaller, representing an additional 13-18% contribution on top of that from CO 2 itself

  2. Performance Evaluation of Blind Tropospheric Delay correction ...

    African Journals Online (AJOL)

    lekky

    and Temperature 2 wet (GPT2w) models) for tropospheric delay correction, ... In practice, a user often employs a certain troposphere model based on the popularity ... comparisons between some of the models have been carried out in the past for .... prediction of meteorological parameter values, which are then used to ...

  3. Homepage for the Global Tropospheric Experiment

    Science.gov (United States)

    Ward, Eugene

    1995-01-01

    The objective of my NASA summer research project was to create a homepage to describe and present results from the NASA Global Tropospheric Experiment (GTE). The GTE is a major component of NASA's Tropospheric Chemistry Program and is managed in the Atmospheric Studies Branch, Atmospheric Sciences Division at the NASA Langley Research Center.

  4. A zonally symmetric model for the monsoon-Hadley circulation with stochastic convective forcing

    Science.gov (United States)

    De La Chevrotière, Michèle; Khouider, Boualem

    2017-02-01

    Idealized models of reduced complexity are important tools to understand key processes underlying a complex system. In climate science in particular, they are important for helping the community improve our ability to predict the effect of climate change on the earth system. Climate models are large computer codes based on the discretization of the fluid dynamics equations on grids of horizontal resolution in the order of 100 km, whereas unresolved processes are handled by subgrid models. For instance, simple models are routinely used to help understand the interactions between small-scale processes due to atmospheric moist convection and large-scale circulation patterns. Here, a zonally symmetric model for the monsoon circulation is presented and solved numerically. The model is based on the Galerkin projection of the primitive equations of atmospheric synoptic dynamics onto the first modes of vertical structure to represent free tropospheric circulation and is coupled to a bulk atmospheric boundary layer (ABL) model. The model carries bulk equations for water vapor in both the free troposphere and the ABL, while the processes of convection and precipitation are represented through a stochastic model for clouds. The model equations are coupled through advective nonlinearities, and the resulting system is not conservative and not necessarily hyperbolic. This makes the design of a numerical method for the solution of this system particularly difficult. Here, we develop a numerical scheme based on the operator time-splitting strategy, which decomposes the system into three pieces: a conservative part and two purely advective parts, each of which is solved iteratively using an appropriate method. The conservative system is solved via a central scheme, which does not require hyperbolicity since it avoids the Riemann problem by design. One of the advective parts is a hyperbolic diagonal matrix, which is easily handled by classical methods for hyperbolic equations, while

  5. The Influence of the North Atlantic Oscillation on Tropospheric Distributions of Ozone and Carbon Monoxide.

    Science.gov (United States)

    Knowland, K. E.; Doherty, R. M.; Hodges, K.

    2015-12-01

    The influence of the North Atlantic Oscillation (NAO) on the tropospheric distributions of ozone (O3) and carbon monoxide (CO) has been quantified. The Monitoring Atmospheric Composition and Climate (MACC) Reanalysis, a combined meteorology and composition dataset for the period 2003-2012 (Innes et al., 2013), is used to investigate the composition of the troposphere and lower stratosphere in relation to the location of the storm track as well as other meteorological parameters over the North Atlantic associated with the different NAO phases. Cyclone tracks in the MACC Reanalysis compare well to the cyclone tracks in the widely-used ERA-Interim Reanalysis for the same 10-year period (cyclone tracking performed using the tracking algorithm of Hodges (1995, 1999)), as both are based on the European Centre for Medium-Range Weather Forecasts' (ECMWF) Integrated Forecast System (IFS). A seasonal analysis is performed whereby the MACC reanalysis meteorological fields, O3 and CO mixing ratios are weighted by the monthly NAO index values. The location of the main storm track, which tilts towards high latitudes (toward the Arctic) during positive NAO phases to a more zonal location in the mid-latitudes (toward Europe) during negative NAO phases, impacts the location of both horizontal and vertical transport across the North Atlantic and into the Arctic. During positive NAO seasons, the persistence of cyclones over the North Atlantic coupled with a stronger Azores High promotes strong horizontal transport across the North Atlantic throughout the troposphere. In all seasons, significantly more intense cyclones occur at higher latitudes (north of ~50°C) during the positive phase of the NAO and in the southern mid-latitudes during the negative NAO phase. This impacts the location of stratospheric intrusions within the descending dry airstream behind the associated cold front of the extratropical cyclone and the venting of low-level pollution up into the free troposphere within

  6. Drivers of the tropospheric ozone budget throughout the 21st century under the medium-high climate scenario RCP 6.0

    Science.gov (United States)

    Revell, L. E.; Tummon, F.; Stenke, A.; Sukhodolov, T.; Coulon, A.; Rozanov, E.; Garny, H.; Grewe, V.; Peter, T.

    2015-05-01

    Because tropospheric ozone is both a greenhouse gas and harmful air pollutant, it is important to understand how anthropogenic activities may influence its abundance and distribution through the 21st century. Here, we present model simulations performed with the chemistry-climate model SOCOL, in which spatially disaggregated chemistry and transport tracers have been implemented in order to better understand the distribution and projected changes in tropospheric ozone. We examine the influences of ozone precursor emissions (nitrogen oxides (NOx), carbon monoxide (CO) and volatile organic compounds (VOCs)), climate change (including methane effects) and stratospheric ozone recovery on the tropospheric ozone budget, in a simulation following the climate scenario Representative Concentration Pathway (RCP) 6.0 (a medium-high, and reasonably realistic climate scenario). Changes in ozone precursor emissions have the largest effect, leading to a global-mean increase in tropospheric ozone which maximizes in the early 21st century at 23% compared to 1960. The increase is most pronounced at northern midlatitudes, due to regional emission patterns: between 1990 and 2060, northern midlatitude tropospheric ozone remains at constantly large abundances: 31% larger than in 1960. Over this 70-year period, attempts to reduce emissions in Europe and North America do not have an effect on zonally averaged northern midlatitude ozone because of increasing emissions from Asia, together with the long lifetime of ozone in the troposphere. A simulation with fixed anthropogenic ozone precursor emissions of NOx, CO and non-methane VOCs at 1960 conditions shows a 6% increase in global-mean tropospheric ozone by the end of the 21st century, with an 11 % increase at northern midlatitudes. This increase maximizes in the 2080s and is mostly caused by methane, which maximizes in the 2080s following RCP 6.0, and plays an important role in controlling ozone directly, and indirectly through its

  7. Tropospheric Ozone and Photochemical Smog

    Science.gov (United States)

    Sillman, S.

    2003-12-01

    emitted species, in a process that is driven by sunlight and is accelerated by warm temperatures. This smog is largely the product of gasoline-powered engines (especially automobiles), although coal-fired industry can also generate photochemical smog. The process of photochemical smog formation was first identified by Haagen-Smit and Fox (1954) in association with Los Angeles, a city whose geography makes it particularly susceptible to this type of smog formation. Sulfate aerosols and organic particulates are often produced concurrently with ozone, giving rise to a characteristic milky-white haze associated with this type of air pollution.Today ozone and particulates are recognized as the air pollutants that are most likely to affect human health adversely. In the United States, most major metropolitan areas have periodic air pollution events with ozone in excess of government health standards. Violations of local health standards also occur in major cities in Canada and in much of Europe. Other cities around the world (especially Mexico City) also experience very high ozone levels. In addition to urban-scale events, elevated ozone occurs in region-wide events in the eastern USA and in Western Europe, with excess ozone extending over areas of 1,000 km2 or more. Ozone plumes of similar extent are found in the tropics (especially in Central Africa) at times of high biomass burning (e.g., Jenkins et al., 1997; Chatfield et al., 1998). In some cases ozone associated with biomass burning has been identified at distances up to 104 km from its sources (Schultz et al., 1999).Ozone also has a significant impact on the global troposphere, and ozone chemistry is a major component of global tropospheric chemistry. Global background ozone concentrations are much lower than urban or regional concentrations during pollution events, but there is evidence that the global background has increased as a result of human activities (e.g., Wang and Jacob, 1998; Volz and Kley, 1988). A rise in

  8. The effect of clouds on photolysis rates and ozone formation in the unpolluted troposphere

    Science.gov (United States)

    Thompson, A. M.

    1984-01-01

    The photochemistry of the lower atmosphere is sensitive to short- and long-term meteorological effects; accurate modeling therefore requires photolysis rates for trace gases which reflect this variability. As an example, the influence of clouds on the production of tropospheric ozone has been investigated, using a modification of Luther's two-stream radiation scheme to calculate cloud-perturbed photolysis rates in a one-dimensional photochemical transport model. In the unpolluted troposphere, where stratospheric inputs of odd nitrogen appear to represent the photochemical source of O3, strong cloud reflectance increases the concentration of NO in the upper troposphere, leading to greatly enhanced rates of ozone formation. Although the rate of these processes is too slow to verify by observation, the calculation is useful in distinguishing some features of the chemistry of regions of differing mean cloudiness.

  9. Convectively driven decadal zonal accelerations in Earth's fluid core

    Science.gov (United States)

    More, Colin; Dumberry, Mathieu

    2018-04-01

    Azimuthal accelerations of cylindrical surfaces co-axial with the rotation axis have been inferred to exist in Earth's fluid core on the basis of magnetic field observations and changes in the length-of-day. These accelerations have a typical timescale of decades. However, the physical mechanism causing the accelerations is not well understood. Scaling arguments suggest that the leading order torque averaged over cylindrical surfaces should arise from the Lorentz force. Decadal fluctuations in the magnetic field inside the core, driven by convective flows, could then force decadal changes in the Lorentz torque and generate zonal accelerations. We test this hypothesis by constructing a quasi-geostrophic model of magnetoconvection, with thermally driven flows perturbing a steady, imposed background magnetic field. We show that when the Alfvén number in our model is similar to that in Earth's fluid core, temporal fluctuations in the torque balance are dominated by the Lorentz torque, with the latter generating mean zonal accelerations. Our model reproduces both fast, free Alfvén waves and slow, forced accelerations, with ratios of relative strength and relative timescale similar to those inferred for the Earth's core. The temporal changes in the magnetic field which drive the time-varying Lorentz torque are produced by the underlying convective flows, shearing and advecting the magnetic field on a timescale associated with convective eddies. Our results support the hypothesis that temporal changes in the magnetic field deep inside Earth's fluid core drive the observed decadal zonal accelerations of cylindrical surfaces through the Lorentz torque.

  10. Dynamics of zonal shear collapse with hydrodynamic electrons

    Science.gov (United States)

    Hajjar, R. J.; Diamond, P. H.; Malkov, M. A.

    2018-06-01

    This paper presents a theory for the collapse of the edge zonal shear layer, as observed at the density limit at low β. This paper investigates the scaling of the transport and mean profiles with the adiabaticity parameter α, with special emphasizes on fluxes relevant to zonal flow (ZF) generation. We show that the adiabaticity parameter characterizes the strength of production of zonal flows and so determines the state of turbulence. A 1D reduced model that self-consistently describes the spatiotemporal evolution of the mean density n ¯ , the azimuthal flow v¯ y , and the turbulent potential enstrophy ɛ=⟨(n˜ -∇2ϕ˜ ) 2/2 ⟩ —related to fluctuation intensity—is presented. Quasi-linear analysis determines how the particle flux Γn and vorticity flux Π=-χy∇2vy+Πre s scale with α, in both hydrodynamic and adiabatic regimes. As the plasma response passes from adiabatic (α > 1) to hydrodynamic (α y=Πre s/χy —representative of the strength of the shear—also drops. The shear layer then collapses and turbulence is enhanced. The collapse is due to a decrease in ZF production, not an increase in damping. A physical picture for the onset of collapse is presented. The findings of this paper are used to motivate an explanation of the phenomenology of low β density limit evolution. A change from adiabatic ( α=kz2vth 2/(|ω|νei)>1 ) to hydrodynamic (α < 1) electron dynamics is associated with the density limit.

  11. Tropospheric radiowave propagation beyond the horizon

    CERN Document Server

    Du Castel, François

    1966-01-01

    Tropospheric Radiowave Propagation Beyond the Horizon deals with developments concerning the tropospheric propagation of ultra-short radio waves beyond the horizon, with emphasis on the relationship between the theoretical and the experimental. Topics covered include the general conditions of propagation in the troposphere; general characteristics of propagation beyond the horizon; and attenuation in propagation. This volume is comprised of six chapters and begins with a brief historical look at the various stages that have brought the technique of transhorizon links to its state of developmen

  12. Forces on zonal flows in tokamak core turbulence

    International Nuclear Information System (INIS)

    Hallatschek, K.; Itoh, K.

    2005-01-01

    The saturation of stationary zonal flows (ZF) in the core of a tokamak has been analyzed in numerical fluid turbulence computer studies. The model was chosen to properly represent the kinetic global plasma flows, i.e., undamped stationary toroidal or poloidal flows and Landau damped geodesic acoustic modes. Reasonable agreement with kinetic simulations in terms of magnitude of transport and occurrence of the Dimits shift was verified. Contrary to common perception, in the final saturated state of turbulence and ZFs, the customary perpendicular Reynolds stress continues to drive the ZFs. The force balance is established by the essentially quasilinear parallel Reynolds stress acting on the parallel return flows required by incompressibility. (author)

  13. Stratospheric Ozone Distribution and Tropospheric General Circulation: Interconnections in the UTLS Region

    Science.gov (United States)

    Barodka, S.; Krasovsky, A.; Shalamyansky, A.

    2014-12-01

    The height of the tropopause, which divided the stratosphere and the troposphere, is a result of two rival categories of processes: the tropospheric vertical convection and the radiative heating of the stratosphere resulting from the ozone cycle. Hence, it is natural that tropospheric and stratospheric phenomena can have effect each other in manifold processes of stratosphere-troposphere interactions. In the present study we focus our attention to the "top-down" side of the interaction: the impact of stratospheric ozone distribution on the features of tropospheric circulation and the associated weather patterns and regional climate conditions. We proceed from analyzes of the observational data performed at the A.I. Voeikov Main Geophysical Observatory, which suggest a distinct correlation between stratospheric ozone distribution, synoptic formations and air-masses boundaries in the upper troposphere and the temperature field of the lower stratosphere [1]. Furthermore, we analyze local features of atmospheric general circulation and stratospheric ozone distribution from the atmospheric reanalyses and general circulation model data, focusing our attention to instantaneous positions of subtropical and polar stationary atmospheric fronts, which define regional characteristics of the general circulation cells in the troposphere and separate global tropospheric air-masses, correspond to distinct meteorological regimes in the TOC field [2, 3]. We assume that by altering the tropopause height, stratospheric ozone-related processes can have an impact on the location of the stationary atmospheric fronts, thereby exerting influence on circulation processes in troposphere and lower stratosphere. For midlatitudes, the tropopause height controls the position of the polar stationary front, which has a direct impact on the trajectory of motion of active vortices on synoptic tropospheric levels, thereby controlling weather patterns in that region and the regional climate. This

  14. A comprehensive spectral theory of zonal-mode dynamics in trapped electron mode turbulence

    International Nuclear Information System (INIS)

    Terry, P.W.; Gatto, R.; Baver, D.A.; Fernandez, E.

    2005-01-01

    A comprehensive, self-consistent theory for spectral dynamics in trapped electron mode (TEM) turbulence offers critical new understanding and insights into zonal-mode physics. This theory shows that 1) zonal mode structure, anisotropy, excitation, and temporal behavior arise at and from the interface of nonlinear advection and linear wave properties; 2) waves induce a marked spectral energy-transfer anisotropy that preferentially drives zonal modes relative to non zonal modes; 3) triplet correlations involving density (as opposed to those involving only flow) mediate the dominant energy transfer at long wavelengths; 4) energy transfer becomes inverse in the presence of wave anisotropy, where otherwise it is forward; 5) zonal-mode excitation is accompanied by excitation of a spectrum of damped eigenmodes, making zonal modes nonlinearly damped; and 6) the combination of anisotropic transfer to zonal modes and their nonlinear damping make this the dominant saturation mechanism for TEM turbulence. This accounts for the reduction of turbulence level by zonal modes, not zonal-flow ExB shearing. (author)

  15. Dynamics of zonal flows and self-regulating drift-wave turbulence

    International Nuclear Information System (INIS)

    Diamond, P.H.; Fleischer, J.; Rosenbluth, M.N.; Hinton, F.L.; Malkov, M.; Smolyakov, A.

    1999-01-01

    We present a theory of zonal flow - drift wave dynamics. Zonal flows are generated by modulational instability of a drift wave spectrum, and are damped by collisions. Drift waves undergo random shearing-induced refraction, resulting in increased mean square radial wavenumber. Drift waves and zonal flows together form a simple dynamical system, which has a single stable fixed point. In this state, the fluctuation intensity and turbulent diffusivity are ultimately proportional to the collisional zonal flow damping. The implications of these results for transport models is discussed. (author)

  16. Dynamics of zonal flows and self-regulating drift-wave turbulence

    International Nuclear Information System (INIS)

    Diamond, P.H.; Fleischer, J.; Rosenbluth, M.; Hinton, F.L.; Malkov, M.; Smolyakov, A.

    2001-01-01

    We present a theory of zonal flow - drift wave dynamics. Zonal flows are generated by modulational instability of a drift wave spectrum, and are damped by collisions. Drift waves undergo random shearing-induced refraction, resulting in increased mean square radial wavenumber. Drift waves and zonal flows together form a simple dynamical system, which has a single stable fixed point. In this state, the fluctuation intensity and turbulent diffusivity are ultimately proportional to the collisional zonal flow damping. The implications of these results for transport models is discussed. (author)

  17. A zonal wavefront sensor with multiple detector planes

    Science.gov (United States)

    Pathak, Biswajit; Boruah, Bosanta R.

    2018-03-01

    A conventional zonal wavefront sensor estimates the wavefront from the data captured in a single detector plane using a single camera. In this paper, we introduce a zonal wavefront sensor which comprises multiple detector planes instead of a single detector plane. The proposed sensor is based on an array of custom designed plane diffraction gratings followed by a single focusing lens. The laser beam whose wavefront is to be estimated is incident on the grating array and one of the diffracted orders from each grating is focused on the detector plane. The setup, by employing a beam splitter arrangement, facilitates focusing of the diffracted beams on multiple detector planes where multiple cameras can be placed. The use of multiple cameras in the sensor can offer several advantages in the wavefront estimation. For instance, the proposed sensor can provide superior inherent centroid detection accuracy that can not be achieved by the conventional system. It can also provide enhanced dynamic range and reduced crosstalk performance. We present here the results from a proof of principle experimental arrangement that demonstrate the advantages of the proposed wavefront sensing scheme.

  18. Zonal structure of unbounded external-flow and aerodynamics

    Energy Technology Data Exchange (ETDEWEB)

    Liu, L Q; Kang, L L; Wu, J Z, E-mail: lqliu@pku.edu.cn [State Key Laboratory of Turbulence and Complex System, Center for Applied Physics and Technology, College of Engineering, Peking University, Beijing 100871 (China)

    2017-08-15

    This paper starts from the far-field behaviors of velocity field in externally unbounded flow. We find that the well-known algebraic decay of disturbance velocity as derived kinematically is too conservative. Once the kinetics are taken into account by working on the fundamental solutions of far-field linearized Navier–Stokes equations, it is proven that the furthest far-field zone adjacent to the uniform fluid at infinity must be unsteady, viscous and compressible, where all disturbances degenerate to sound waves that decay exponentially. But this optimal rate does not exist in some commonly used simplified flow models, such as steady flow, incompressible flow and inviscid flow, because they actually work in true subspaces of the unbounded free space, which are surrounded by further far fields of different nature. This finding naturally leads to a zonal structure of externally unbounded flow field. The significance of the zonal structure is demonstrated by its close relevance to existing theories of aerodynamic force and moment in external flows, including the removal of the difficulties or paradoxes inherent in the simplified models. (paper)

  19. The use of satellite data to determine the distribution of ozone in the troposphere

    Science.gov (United States)

    Fishman, Jack; Watson, Catherine E.; Brackett, Vincent G.; Fakhruzzaman, Khan; Veiga, Robert E.

    1991-01-01

    Measurements from two independent satellite data sets have been used to derive the climatology of the integrated amount of ozone in the troposphere. These data have led to the finding that large amounts of ozone pollution are generated by anthropogenic activity originating from both the industrialized regions of the Northern Hemisphere and from the southern tropical regions of Africa. To verify the existence of this ozone anomaly at low latitudes, an ozonesonde capability has been established at Ascension Island (8 deg S, 15 deg W) since July 1990. According to the satellite analyses, Ascension Island is located downwind of the primary source region of this ozone pollution, which likely results from the photochemical oxidation of emissions emanating from the widespread burning of savannas and other biomass. These in situ measurements confirm the existence of large amounts of ozone in the lower atmosphere. A summary of these ozonesonde data to date will be presented. In addition, we will present some ozone profile measurements from SAGE II which can be used to provide upper tropospheric ozone measurements directly in the tropical troposphere. A preliminary comparison between the satellite observations and the ozonesonde profiles in the upper troposphere and lower stratosphere will also be presented.

  20. Concentration variations of the tropospheric carbon dioxide over the Antarctic region

    Directory of Open Access Journals (Sweden)

    Shohei Murayama

    1997-03-01

    Full Text Available Aircraft measurements of the atmospheric CO_2 concentration have been made over Syowa Station, Antarctica since 1983. The minimum concentration of the average seasonal CO_2 cycle appears in March throughout the troposphere, while the maximum concentration occurs in mid-August in the upper troposphere and in late September in the middle and lower troposphere. The peak-to-peak amplitude of the seasonal cycle decreases with height. The CO_2 concentration increases with height during most of the year; however, this height dependency is larger from summer to early winter than in the remaining seasons. The average concentration difference between the upper troposphere and the ground surface is about 0.3ppmv. From comparisons with the results of the ground-based and aircraft measurements at southern middle and high latitudes and trajectory analysis, it is hypothesized that the seasonal cycle of height-dependent atmospheric transport processes could influence the seasonal cycle and the vertical distribution of the CO_2 concentration over Syowa Station.

  1. Southern Hemisphere Carbon Monoxide Inferannual Variability Observed by Terra/Measurement of Pollution in the Troposphere (MOPITT)

    Science.gov (United States)

    Edwards, D. P.; Petron, G.; Novelli, P. C.; Emmons, L. K.; Gille, J. C.; Drummond, J. R.

    2010-01-01

    Biomass burning is an annual occurrence in the tropical southern hemisphere (SH) and represents a major source of regional pollution. Vegetation fires emit carbon monoxide (CO), which due to its medium lifetime is an excellent tracer of tropospheric transport. CO is also one of the few tropospheric trace gases currently observed from satellite and this provides long-term global measurements. In this paper, we use the 5 year CO data record from the Measurement Of Pollution In The Troposphere (MOPITT) instrument to examine the inter-annual variability of the SH CO loading and show how this relates to climate conditions which determine the intensity of fire sources. The MOPITT observations show an annual austral springtime peak in the SH zonal CO loading each year with dry-season biomass burning emissions in S. America, southern Africa, the Maritime Continent, and northwestern Australia. Although fires in southern Africa and S. America typically produce the greatest amount of CO, the most significant inter-annual variation is due to varying fire activity and emissions from the Maritime Continent and northern Australia. We find that this variation in turn correlates well with the El Nino Southern Oscillation precipitation index. Between 2000 and 2005, emissions were greatest in late 2002 and an inverse modeling of the MOPITT data using the MOZART chemical transport model estimates the southeast Asia regional fire source for the year August 2002 to September 2003 to be 52 Tg CO. Comparison of the MOPITT retrievals and NOAA surface network measurements indicate that the latter do not fully capture the inter-annual variability or the seasonal range of the CO zonal average concentration due to biases associated with atmospheric and geographic sampling.

  2. Tropospheric ozone changes, radiative forcing and attribution to emissions in the Atmospheric Chemistry and Climate Model Intercomparison Project (ACCMIP

    Directory of Open Access Journals (Sweden)

    D. S. Stevenson

    2013-03-01

    : decreases in the tropical lower troposphere, associated with increases in water vapour; and increases in the sub-tropical to mid-latitude upper troposphere, associated with increases in lightning and stratosphere-to-troposphere transport. Climate change has relatively small impacts on global mean tropospheric ozone RF.

  3. Spatial variability of the structure of the lower troposphere over north western Indian Ocean during 1983 summer monsoon

    Digital Repository Service at National Institute of Oceanography (India)

    RameshKumar, M.R.; Sadhuram, Y.; Michael, G.S.; Rao, L.V.G.

    The spatial variability of the structure of the lower troposphere over the north western Indian Ocean during the period 12th July to 2nd September, 1983 has been studied using the upper air data collected during the first scientific cruise of @i...

  4. The application of zonal trademark combustion monitoring and tuning system to coal boilers for efficiency improvement and emissions reduction

    Energy Technology Data Exchange (ETDEWEB)

    Xu, Guang; Zhou, Wei; Widmer, Neil C.; Moyeda, David K. [GE Energy, Irvine, CA (United States)

    2013-07-01

    Coal-fired boilers equipped with Low NO{sub x} Burner (LNB) and Overfire Air (OFA) are challenged with maintaining good combustion conditions. In many cases, the significant increases in carbon monoxide (CO) and unburned carbon levels can be attributed to local poor combustion conditions as a result of poorly controlled fuel-air distribution within the furnace. The Zonal trademark combustion monitoring and tuning system developed by GE is available to detect and correct the furnace air-fuel distribution imbalance. The system monitors the boiler excess oxygen (O{sub 2}) and combustible gases, primarily carbon monoxide (CO), by using spatially distributed multipoint sensors located in the boiler's high temperature upper convective backpass region. At these locations, the furnace flow is still significantly stratified allowing tracing of poor combustion zones to specific burners and OFA ports. Using a model-based tuning system, operators can rapidly respond to poor combustion conditions by redistributing airflows to select burners and OFA ports. By improving combustion at every point within the furnace, the boiler can operate at reduced excess O{sub 2} and reduced furnace exit gas temperature (FEGT) while also reducing localized hot spots, corrosive gas conditions, slag formation, and carbon-in-ash. Benefits include improving efficiency, reducing NO{sub X} emissions, increasing output and maximizing availability. This chapter presents the results from implementing the Zonal combustion monitoring and tuning system on a 460 MW tangential-fired coal boiler in the Western United States.

  5. Acute Zonal Occult Outer Retinopathy with Atypical Findings

    Directory of Open Access Journals (Sweden)

    Dimitrios Karagiannis

    2014-01-01

    Full Text Available Background. To report a case of acute zonal occult outer retinopathy (AZOOR with atypical electrophysiology findings. Case Presentation. A 23-year-old-female presented with visual acuity deterioration in her right eye accompanied by photopsia bilaterally. Corrected distance visual acuity at presentation was 20/50 in the right eye and 20/20 in the left eye. Fundus examination was unremarkable. Visual field (VF testing revealed a large scotoma. Pattern and full-field electroretinograms (PERG and ERG revealed macular involvement associated with generalized retinal dysfunction. Electrooculogram (EOG light rise and the Arden ratio were within normal limits bilaterally. The patient was diagnosed with AZOOR due to clinical findings, visual field defect, and ERG findings. Conclusion. This is a case of AZOOR with characteristic VF defects and clinical symptoms presenting with atypical EOG findings.

  6. A zonal Galerkin-free POD model for incompressible flows

    Science.gov (United States)

    Bergmann, Michel; Ferrero, Andrea; Iollo, Angelo; Lombardi, Edoardo; Scardigli, Angela; Telib, Haysam

    2018-01-01

    A domain decomposition method which couples a high and a low-fidelity model is proposed to reduce the computational cost of a flow simulation. This approach requires to solve the high-fidelity model in a small portion of the computational domain while the external field is described by a Galerkin-free Proper Orthogonal Decomposition (POD) model. We propose an error indicator to determine the extent of the interior domain and to perform an optimal coupling between the two models. This zonal approach can be used to study multi-body configurations or to perform detailed local analyses in the framework of shape optimisation problems. The efficiency of the method to perform predictive low-cost simulations is investigated for an unsteady flow and for an aerodynamic shape optimisation problem.

  7. Combining zonal refractive and diffractive aspheric multifocal intraocular lenses.

    Science.gov (United States)

    Muñoz, Gonzalo; Albarrán-Diego, César; Javaloy, Jaime; Sakla, Hani F; Cerviño, Alejandro

    2012-03-01

    To assess visual performance with the combination of a zonal refractive aspheric multifocal intraocular lens (MIOL) (Lentis Mplus, Oculentis GmbH) and a diffractive aspheric MIOL (Acri.Lisa 366, Acri.Tech GmbH). This prospective interventional cohort study comprised 80 eyes from 40 cataract patients (mean age: 65.5±7.3 years) who underwent implantation of the Lentis Mplus MIOL in one eye and Acri.Lisa 366 MIOL in the fellow eye. The main outcome measures were refraction; monocular and binocular uncorrected and corrected distance, intermediate, and near visual acuities; monocular and binocular defocus curves; binocular photopic contrast sensitivity function compared to a monofocal intraocular lens (IOL) control group (40 age-matched pseudophakic patients implanted with the AR-40e [Abbott Medical Optics]); and quality of vision questionnaire. Binocular uncorrected visual acuities were 0.12 logMAR (0.76 decimal) or better at all distances measured between 6 m and 33 cm. The Lentis Mplus provided statistically significant better vision than the Acri.Lisa at distances between 2 m and 40 cm, and the Acri.Lisa provided statistically significant better vision than the Lentis Mplus at 33 cm. Binocular defocus curve showed little drop-off at intermediate distances. Photopic contrast sensitivity function for distance and near were similar to the monofocal IOL control group except for higher frequencies. Moderate glare (15%), night vision problems (12.5%), and halos (10%) were reported. Complete independence of spectacles was achieved by 92.5% of patients. The combination of zonal refractive aspheric and diffractive aspheric MIOLs resulted in excellent uncorrected binocular distance, intermediate, and near vision, with low incidence of significant photic phenomena and high patient satisfaction. Copyright 2012, SLACK Incorporated.

  8. SPI Conformance Gel Applications in Geothermal Zonal Isolation

    Energy Technology Data Exchange (ETDEWEB)

    Burns, Lyle [Clean Tech Innovations, Bartlesville, OK (United States)

    2017-08-08

    Zonal isolation in geothermal injection and producing wells is important while drilling the wells when highly fractured geothermal zones are encountered and there is a need to keep the fluids from interfering with the drilling operation. Department of Energy’s (DOE) Energy Efficiency and Renewable Energy (EERE) objectives are to advance technologies to make it more cost effective to develop, produce, and monitor geothermal reservoirs and produce geothermal energy. Thus, zonal isolation is critical to well cost, reservoir evaluation and operations. Traditional cementing off of the lost circulation or thief zones during drilling is often done to stem the drilling mud losses. This is an expensive and generally unsuccessful technique losing the potential of the remaining fracture system. Selective placement of strong SPI gels into only the offending fractures can maintain and even improve operational efficiency and resource life. The SPI gel system is a unique silicate based gel system that offers a promising solution to thief zones and conformance problems with water and CO2 floods and potentially geothermal operations. This gel system remains a low viscosity fluid until an initiator (either internal such as an additive or external such as CO2) triggers gelation. This is a clear improvement over current mechanical methods of using packers, plugs, liners and cementing technologies that often severely damage the highly fractured area that is isolated. In the SPI gels, the initiator sets up the fluid into a water-like (not a precipitate) gel and when the isolated zone needs to be reopened, the SPI gel may be removed with an alkaline solution without formation damage occurring. In addition, the SPI gel in commercial quantities is expected to be less expensive than competing mechanical systems and has unique deep placement possibilities. This project seeks to improve upon the SPI gel integrity by modifying the various components to impart temperature stability for use in

  9. Identification of zonal flows and their characteristics on transport barrier in CHS

    International Nuclear Information System (INIS)

    Fujisawa, A.; Shimizu, A.; Nakano, H.; Ohshima, S.; Iguchi, H.; Yoshimura, Y.; Minami, T.; Itoh, K.; Isobe, M.; Suzuki, C.; Nishimura, S.; Akiyama, T.; Nagaoka, K.; Takahashi, C.; Ida, K.; Toi, K.; Okamura, S.; Matsuoka, K.; Itoh, S.-I.; Diamond, P.H.

    2005-01-01

    Relation between turbulence and electric field has been one of the central issues related to the transport physics of toroidal plasmas. Recently, zonal flow, axi-symmetric band-like structure (m=n=0) with a finite radial wavelength, has just come up the third element responsible for the plasma transport. Theories and simulations have expected that the zonal flow should be a mechanism to control the saturation level of turbulence and the resultant transport. In CHS, dual heavy ion beam probes (HIBP) succeeded to prove the presence of the zonal flow and to show the dynamics and structure of the zonal flows. The experiment shows a long-distance correlation between radial electric field (or plasma flow) in low frequency range (< ∼1 kHz), together with radial structure of the zonal flow; characteristic radial length of ∼1.5 cm and life time of ∼1.5 ms. Different characteristics of the zonal flow and turbulence was found in states with and without a transport barrier; the zonal flow activity shrinks with an increase in turbulence level after the barrier breaks down. The recent HIBP experiments have just provided further insight into the system of zonal flow and turbulence. A wavelet analysis is performed on the fluctuation on the barrier position in the state with the transport barrier. The analysis reveals a causal relationship between the zonal flow evolution and turbulence level; the zonal flow is found to increase toward the mean flow direction as turbulence level decreases in the frequency range of 100-150kHz. The observation shows the presence of a nonlinear interaction between zonal flow and the turbulence, or a process of the zonal flow to affect the turbulence level. This paper presents surveys on zonal flow, particularly the recent experiments to demonstrate a causal relationship between zonal flow component and turbulence. Besides, other results obtained with a wavelet analysis are presented on the transport barrier; e.g., density and potential

  10. Change of Zonal Flow Spectra in the JIPP T-IIU Tokamak Plasmas

    International Nuclear Information System (INIS)

    Hamada, Y.; Watari, T.; Yamagishi, O.; Nishizawa, A.; Narihara, K.; Kawasumi, Y.; Ido, T.; Kojima, M.; Toi, K.

    2007-01-01

    When Ohmically heated low-density plasmas are additionally heated by higher-harmonics ion-cyclotron-range-of frequency heating, heated by neutral beam injection, or strongly gas puffed, the intensity of zonal flows in the geodesic acoustic mode frequency range in the tokamak core plasma decreases sharply and that of low-frequency zonal flow grows drastically. This is accompanied by a damping of the drift wave propagating in the electron diamagnetic drift direction, turbulence by trapped electron mode (TEM), and the increase of the mode propagating to ion diamagnetic drift direction (ITG). In the half-radius region, TEM and high-frequency zonal flows remain intense in both OH and heated phases. ITG and low-frequency zonal flows grow in heated plasmas, suggesting a strong coupling between ITG and low-frequency zonal flow

  11. GOZCARDS Source Data for Ozone Monthly Zonal Means on a Geodetic Latitude and Pressure Grid V1.01

    Data.gov (United States)

    National Aeronautics and Space Administration — The GOZCARDS Source Data for Ozone Monthly Zonal Averages on a Geodetic Latitude and Pressure Grid product (GozSmlpO3) contains zonal means and related information...

  12. GOZCARDS Source Data for Nitrous Oxide Monthly Zonal Means on a Geodetic Latitude and Pressure Grid V1.01

    Data.gov (United States)

    National Aeronautics and Space Administration — The GOZCARDS Source Data for Nitrous Oxide Monthly Zonal Averages on a Geodetic Latitude and Pressure Grid product (GozSmlpN2O) contains zonal means and related...

  13. GOZCARDS Source Data for Temperature Monthly Zonal Averages on a Geodetic Latitude and Pressure Grid V1.00

    Data.gov (United States)

    National Aeronautics and Space Administration — The GOZCARDS Source Data for Temperature Monthly Zonal Averages on a Geodetic Latitude and Pressure Grid product (GozSmlpT) contains zonal means and related...

  14. GOZCARDS Source Data for Nitric Acid Monthly Zonal Means on a Geodetic Latitude and Pressure Grid V1.01

    Data.gov (United States)

    National Aeronautics and Space Administration — The GOZCARDS Source Data for Nitric Acid Monthly Zonal Averages on a Geodetic Latitude and Pressure Grid product (GozSmlpHNO3) contains zonal means and related...

  15. NOAA Climate Data Record (CDR) of Zonal Mean Ozone Binary Database of Profiles (BDBP), version 1.0

    Data.gov (United States)

    National Oceanic and Atmospheric Administration, Department of Commerce — This NOAA Climate Data Record (CDR) of Zonal Mean Ozone Binary Database of Profiles (BDBP) dataset is a vertically resolved, global, gap-free and zonal mean dataset...

  16. GOZCARDS Merged Data for Nitrous Oxide Monthly Zonal Means on a Geodetic Latitude and Pressure Grid V1.01

    Data.gov (United States)

    National Aeronautics and Space Administration — The GOZCARDS Merged Data for Nitrous Oxide Monthly Zonal Averages on a Geodetic Latitude and Pressure Grid product (GozMmlpN2O) contains zonal means and related...

  17. GOZCARDS Merged Data for Water Vapor Monthly Zonal Means on a Geodetic Latitude and Pressure Grid V1.01

    Data.gov (United States)

    National Aeronautics and Space Administration — The GOZCARDS Merged Data for Water Vapor Monthly Zonal Averages on a Geodetic Latitude and Pressure Grid product (GozMmlpH2O) contains zonal means and related...

  18. GOZCARDS Merged Data for Hydrogen Chloride Monthly Zonal Means on a Geodetic Latitude and Pressure Grid V1.01

    Data.gov (United States)

    National Aeronautics and Space Administration — The GOZCARDS Merged Data for Hydrogen Chloride Monthly Zonal Averages on a Geodetic Latitude and Pressure Grid product (GozMmlpHCl) contains zonal means and related...

  19. GOZCARDS Merged Data for Ozone Monthly Zonal Means on a Geodetic Latitude and Pressure Grid V1.01

    Data.gov (United States)

    National Aeronautics and Space Administration — The GOZCARDS Merged Data for Ozone Monthly Zonal Averages on a Geodetic Latitude and Pressure Grid product (GozMmlpO3) contains zonal means and related information...

  20. GOZCARDS Merged Data for Nitric Acid Monthly Zonal Means on a Geodetic Latitude and Pressure Grid V1.01

    Data.gov (United States)

    National Aeronautics and Space Administration — The GOZCARDS Merged Data for Nitric Acid Monthly Zonal Averages on a Geodetic Latitude and Pressure Grid product (GozMmlpHNO3) contains zonal means and related...

  1. Upper-Level Waves of Synoptic Scale at Midlatitudes

    Science.gov (United States)

    Rivest, Chantal

    1990-01-01

    Upper-level waves of synoptic scale are important dynamical entities at midlatitudes. They often induce surface cyclogenesis (cf. Peterssen and Smebye, 1971), and their life duration is typically longer than time scales for disruption by the ambient shear (Sanders, 1988). The objectives of the present thesis are to explain the maintenance and genesis of upper-level synoptic-scale waves in the midlatitude flow. We develop an analytical model of waves on generalized Eady basic states that have uniform tropospheric and stratospheric potential vorticity, but allow for the decay of density with height. The Eady basic state represents the limiting case of infinite stratospheric stability and constant density. We find that the Eady normal mode characteristics hold in the presence of realistic tropopause and stratosphere. In particular, the basic states studied support at the synoptic scale upper-level normal modes. These modes provide simple models for the dynamics of upper-level synoptic-scale waves, as waves supported by the large latitudinal gradients of potential vorticity at the tropopause. In the presence of infinitesimal positive tropospheric gradients of potential vorticity, the upper-level normal mode solutions no longer exist, as was demonstrated in Green (1960). Disappearance of the normal mode solution when a parameter changes slightly represents a dilemma that we seek to understand. We examine what happens to the upper-level normal modes in the presence of tropospheric gradients of potential vorticity in a series of initial -value experiments. Our results show that the normal modes become slowly decaying quasi-modes. Mathematically the quasi-modes consist of a superposition of singular modes sharply peaked in the phase speed domain, and their decay proceeds as the modes interfere with one another. We repeat these experiments in basic states with a smooth tropopause in the presence of tropospheric and stratospheric gradients, and similar results are obtained

  2. Tropospheric VOC measurements by PTR-MS

    International Nuclear Information System (INIS)

    Hansel, A.; Wisthaler, A.; Graus, M.; Grabmer, W.

    2002-01-01

    Full text: O 3 is formed photochemically from the photolysis of NO 2 , and because O 3 reacts rapidly with NO these reactions result in a photoequilibrium between NO, NO 2 with no net formation or loss of O 3 , However, in the presence of volatile organic compounds (VOCs), the degradation reactions of VOCs lead to the formation of intermediate peroxy radicals which react with NO, converting NO to NO 2 , which then photolyze to form O 3 . Thus, in order to understand quantitatively tropospheric ozone chemistry, it is necessary to know the VOC distribution within the troposphere as well as VOC fluxes from individual sources. Examples will be presented how the use of Proton Transfer Reaction Mass Spectrometry (PTR-MS) has enhanced our understanding of anthropogenic VOC emissions, biosphere-atmosphere exchange processes, and photochemical processing of both anthropogenic and biogenic VOCs in the troposphere. (author)

  3. Intra-seasonal Oscillations (ISO of zonal-mean meridional winds and temperatures as measured by UARS

    Directory of Open Access Journals (Sweden)

    F. T. Huang

    2005-06-01

    Full Text Available Based on an empirical analysis of measurements with the High Resolution Doppler Imager (HRDI on the UARS spacecraft in the upper mesosphere (95km, persistent and regular intra-seasonal oscillations (ISO with periods of about 2 to 4 months have recently been reported in the zonal-mean meridional winds. Similar oscillations have also been discussed independently in a modeling study, and they were attributed to wave-mean-flow interactions. The observed and modeled meridional wind ISOs were largely confined to low latitudes. We report here on an analysis of concurrent UARS temperature measurements, which produces oscillations similar to those seen in the meridional winds. Although the temperature oscillations are observed at lower altitudes (55km, their phase variations with latitude are qualitatively consistent with the inferred properties seen in the meridional winds and thus provide independent evidence for the existence of ISOs in the mesosphere.

  4. Applications of Satellite Observations of Tropospheric Composition

    Science.gov (United States)

    Monks, Paul S.; Beirle, Steffen

    A striking feature of the field of tropospheric composition is the sheer number of chemical species that have been detected and measured with satellite instruments. The measurements have found application both in atmospheric chemistry itself, providing evidence, for example, of unexpected cryochemistry in the Arctic regions, and also in environmental monitoring with, for example, the observed growth in NO2 emissions over eastern Asia. Chapter 8 gives an overview of the utility of satellite observations for measuring tropospheric composition, dealing with each of the many compounds seen in detail. A comprehensive compound by compound table of the many studies performed is a most useful feature.

  5. Impact of climate variability on tropospheric ozone

    International Nuclear Information System (INIS)

    Grewe, Volker

    2007-01-01

    A simulation with the climate-chemistry model (CCM) E39/C is presented, which covers both the troposphere and stratosphere dynamics and chemistry during the period 1960 to 1999. Although the CCM, by its nature, is not exactly representing observed day-by-day meteorology, there is an overall model's tendency to correctly reproduce the variability pattern due to an inclusion of realistic external forcings, like observed sea surface temperatures (e.g. El Nino), major volcanic eruption, solar cycle, concentrations of greenhouse gases, and Quasi-Biennial Oscillation. Additionally, climate-chemistry interactions are included, like the impact of ozone, methane, and other species on radiation and dynamics, and the impact of dynamics on emissions (lightning). However, a number of important feedbacks are not yet included (e.g. feedbacks related to biogenic emissions and emissions due to biomass burning). The results show a good representation of the evolution of the stratospheric ozone layer, including the ozone hole, which plays an important role for the simulation of natural variability of tropospheric ozone. Anthropogenic NO x emissions are included with a step-wise linear trend for each sector, but no interannual variability is included. The application of a number of diagnostics (e.g. marked ozone tracers) allows the separation of the impact of various processes/emissions on tropospheric ozone and shows that the simulated Northern Hemisphere tropospheric ozone budget is not only dominated by nitrogen oxide emissions and other ozone pre-cursors, but also by changes of the stratospheric ozone budget and its flux into the troposphere, which tends to reduce the simulated positive trend in tropospheric ozone due to emissions from industry and traffic during the late 80s and early 90s. For tropical regions the variability in ozone is dominated by variability in lightning (related to ENSO) and stratosphere-troposphere exchange (related to Northern Hemisphere Stratospheric

  6. Stratospheric ozone intrusion events and their impacts on tropospheric ozone in the Southern Hemisphere

    Directory of Open Access Journals (Sweden)

    J. W. Greenslade

    2017-09-01

    Full Text Available Stratosphere-to-troposphere transport (STT provides an important natural source of ozone to the upper troposphere, but the characteristics of STT events in the Southern Hemisphere extratropics and their contribution to the regional tropospheric ozone budget remain poorly constrained. Here, we develop a quantitative method to identify STT events from ozonesonde profiles. Using this method we estimate the seasonality of STT events and quantify the ozone transported across the tropopause over Davis (69° S, 2006–2013, Macquarie Island (54° S, 2004–2013, and Melbourne (38° S, 2004–2013. STT seasonality is determined by two distinct methods: a Fourier bandpass filter of the vertical ozone profile and an analysis of the Brunt–Väisälä frequency. Using a bandpass filter on 7–9 years of ozone profiles from each site provides clear detection of STT events, with maximum occurrences during summer and minimum during winter for all three sites. The majority of tropospheric ozone enhancements owing to STT events occur within 2.5 and 3 km of the tropopause at Davis and Macquarie Island respectively. Events are more spread out at Melbourne, occurring frequently up to 6 km from the tropopause. The mean fraction of total tropospheric ozone attributed to STT during STT events is  ∼ 1. 0–3. 5 % at each site; however, during individual events, over 10 % of tropospheric ozone may be directly transported from the stratosphere. The cause of STTs is determined to be largely due to synoptic low-pressure frontal systems, determined using coincident ERA-Interim reanalysis meteorological data. Ozone enhancements can also be caused by biomass burning plumes transported from Africa and South America, which are apparent during austral winter and spring and are determined using satellite measurements of CO. To provide regional context for the ozonesonde observations, we use the GEOS-Chem chemical transport model, which is too coarsely

  7. Spectropolarimetric Measurements of Scattered Sunlight in the Huggins Bands: Retrieval of Tropospheric Ozone Profiles

    Science.gov (United States)

    Fu, D.; Sander, S. P.; Stutz, J.; Pongetti, T. J.; Yung, Y. L.; Wong, M.; Natraj, V.; Li, K.; Shia, R.

    2009-12-01

    Ozone concentrations in the troposphere have increased over the past century as a result of anthropogenic emissions of NOx and volatile organic compounds. In addition to being harmful to human health and plant life, ozone is an important greenhouse gas, especially in the middle and upper troposphere. Therefore, accurate monitoring of tropospheric ozone vertical distributions is crucial for a better understanding of air quality and climate change. Simulations of vector radiative transfer in the near ultraviolet region have shown that tropospheric ozone profiles can be retrieved using polarization measurements. However, to date there has been no experimental test of this method. A new compact, portable spectropolarimeter has been built for atmospheric remote sensing. The first comprehensive description of the configuration and performance of this instrument for ground-based operation is provided and sample atmospheric scattered sunlight spectra are shown. Using optimal estimation retrieval theory we study the information content of polarization spectra in the Huggins band and uncertainties in the retrieval associated with the measurement parameters, such as aerosol scattering.

  8. Turbulence, transport, and zonal flows in the Madison symmetric torus reversed-field pinch

    Science.gov (United States)

    Williams, Z. R.; Pueschel, M. J.; Terry, P. W.; Hauff, T.

    2017-12-01

    The robustness and the effect of zonal flows in trapped electron mode (TEM) turbulence and Ion Temperature Gradient (ITG) turbulence in the reversed-field pinch (RFP) are investigated from numerical solutions of the gyrokinetic equations with and without magnetic external perturbations introduced to model tearing modes. For simulations without external magnetic field perturbations, zonal flows produce a much larger reduction of transport for the density-gradient-driven TEM turbulence than they do for the ITG turbulence. Zonal flows are studied in detail to understand the nature of their strong excitation in the RFP and to gain insight into the key differences between the TEM- and ITG-driven regimes. The zonal flow residuals are significantly larger in the RFP than in tokamak geometry due to the low safety factor. Collisionality is seen to play a significant role in the TEM zonal flow regulation through the different responses of the linear growth rate and the size of the Dimits shift to collisionality, while affecting the ITG only minimally. A secondary instability analysis reveals that the TEM turbulence drives zonal flows at a rate that is twice that of the ITG turbulence. In addition to interfering with zonal flows, the magnetic perturbations are found to obviate an energy scaling relation for fast particles.

  9. Chemical processes related to net ozone tendencies in the free troposphere

    Science.gov (United States)

    Bozem, Heiko; Butler, Tim M.; Lawrence, Mark G.; Harder, Hartwig; Martinez, Monica; Kubistin, Dagmar; Lelieveld, Jos; Fischer, Horst

    2017-09-01

    Ozone (O3) is an important atmospheric oxidant, a greenhouse gas, and a hazard to human health and agriculture. Here we describe airborne in situ measurements and model simulations of O3 and its precursors during tropical and extratropical field campaigns over South America and Europe, respectively. Using the measurements, net ozone formation/destruction tendencies are calculated and compared to 3-D chemistry-transport model simulations. In general, observation-based net ozone tendencies are positive in the continental boundary layer and the upper troposphere at altitudes above ˜ 6 km in both environments. On the other hand, in the marine boundary layer and the middle troposphere, from the top of the boundary layer to about 6-8 km altitude, net O3 destruction prevails. The ozone tendencies are controlled by ambient concentrations of nitrogen oxides (NOx). In regions with net ozone destruction the available NOx is below the threshold value at which production and destruction of O3 balance. While threshold NO values increase with altitude, in the upper troposphere NOx concentrations are generally higher due to the integral effect of convective precursor transport from the boundary layer, downward transport from the stratosphere and NOx produced by lightning. Two case studies indicate that in fresh convective outflow of electrified thunderstorms net ozone production is enhanced by a factor 5-6 compared to the undisturbed upper tropospheric background. The chemistry-transport model MATCH-MPIC generally reproduces the pattern of observation-based net ozone tendencies but mostly underestimates the magnitude of the net tendency (for both net ozone production and destruction).

  10. Assessment of NOAA NUCAPS upper air temperature profiles using COSMIC GPS radio occultation and ARM radiosondes

    Science.gov (United States)

    Feltz, M. L.; Borg, L.; Knuteson, R. O.; Tobin, D.; Revercomb, H.; Gambacorta, A.

    2017-09-01

    The U.S. National Oceanic and Atmospheric Administration (NOAA) recently began operational processing to derive vertical temperature profiles from two new sensors, Cross-Track Infrared Sounder and Advanced Technology Microwave Sounder, which were developed for the next generation of U.S. weather satellites. The NOAA-Unique Combined Atmospheric Processing System (NUCAPS) has been developed by NOAA to routinely process data from future Joint Polar Satellite System operational satellites and the preparatory Suomi-NPP satellite. This paper assesses the NUCAPS vertical temperature profile product from the upper troposphere into the middle stratosphere using radiosonde and GPS radio occultation (RO) data. Radiosonde data from the Department of Energy Atmospheric Radiation Measurement (ARM) program are=] compared to both the NUCAPS and GPS RO temperature products to evaluate bias and RMS errors. At all three fixed ARM sites for time periods investigated the NUCAPS temperature in the 100-40 hPa range is found to have an average bias to the radiosondes of less than 0.45 K and an RMS error of less than 1 K when temperature averaging kernels are applied. At a 95% confidence level, the radiosondes and RO were found to agree within 0.4 K at the North Slope of Alaska site and within 0.83 K at Southern Great Plains and Tropical Western Pacific. The GPS RO-derived dry temperatures, obtained from the University Corporation for Atmospheric Research Constellation Observing System for Meteorology, Ionosphere, and Climate (COSMIC) mission, are used as a common reference for the intercomparison of NUCAPS temperature products to similar products produced by NASA from Atmospheric Infrared Sounder (AIRS) and by European Organisation for the Exploitation of Meteorological Satellites from MetOp-B Infrared Atmospheric Sounding Interferometer (IASI). For seasonal and zonal scales, the NUCAPS agreement with AIRS and IASI is less than 0.5 K after application of averaging kernels.

  11. Fluid simulation of tokamak ion temperature gradient turbulence with zonal flow closure model

    Energy Technology Data Exchange (ETDEWEB)

    Yamagishi, Osamu, E-mail: yamagisi@nifs.ac.jp; Sugama, Hideo [National Institute for Fusion Science, Toki, Gifu 509-5292 (Japan)

    2016-03-15

    Nonlinear fluid simulation of turbulence driven by ion temperature gradient modes in the tokamak fluxtube configuration is performed by combining two different closure models. One model is a gyrofluid model by Beer and Hammett [Phys. Plasmas 3, 4046 (1996)], and the other is a closure model to reproduce the kinetic zonal flow response [Sugama et al., Phys. Plasmas 14, 022502 (2007)]. By including the zonal flow closure, generation of zonal flows, significant reduction in energy transport, reproduction of the gyrokinetic transport level, and nonlinear upshift on the critical value of gradient scale length are observed.

  12. Zonal flow excitation by Shukla-Varma modes in a nonuniform dusty magnetoplasma

    International Nuclear Information System (INIS)

    Shukla, P.K.; Stenflo, L.

    2002-01-01

    The nonlinear coupling between the Shukla-Varma (SV) modes and the zonal flows in a nonuniform dusty magnetoplasma is considered. By using a two-fluid model and the guiding center particle drifts, a pair of coupled mode equations is obtained. The latter are Fourier analyzed to obtain a nonlinear dispersion relation, which exhibits the excitation of zonal flows by the ponderomotive force of the SV modes. The increment of the parametrically excited zonal flows is presented. The relevance of our investigation to laboratory and space plasmas is discussed

  13. Fluid simulation of tokamak ion temperature gradient turbulence with zonal flow closure model

    Science.gov (United States)

    Yamagishi, Osamu; Sugama, Hideo

    2016-03-01

    Nonlinear fluid simulation of turbulence driven by ion temperature gradient modes in the tokamak fluxtube configuration is performed by combining two different closure models. One model is a gyrofluid model by Beer and Hammett [Phys. Plasmas 3, 4046 (1996)], and the other is a closure model to reproduce the kinetic zonal flow response [Sugama et al., Phys. Plasmas 14, 022502 (2007)]. By including the zonal flow closure, generation of zonal flows, significant reduction in energy transport, reproduction of the gyrokinetic transport level, and nonlinear upshift on the critical value of gradient scale length are observed.

  14. Tropospheric Ozone from the TOMS TDOT (TOMS-Direct-Ozone-in-Troposphere) Technique During SAFARI-2000

    Science.gov (United States)

    Stone, J. B.; Thompson, A. M.; Frolov, A. D.; Hudson, R. D.; Bhartia, P. K. (Technical Monitor)

    2002-01-01

    There are a number of published residual-type methods for deriving tropospheric ozone from TOMS (Total Ozone Mapping Spectrometer). The basic concept of these methods is that within a zone of constant stratospheric ozone, the tropospheric ozone column can be computed by subtracting stratospheric ozone from the TOMS Level 2 total ozone column, We used the modified-residual method for retrieving tropospheric ozone during SAFARI-2000 and found disagreements with in-situ ozone data over Africa in September 2000. Using the newly developed TDOT (TOMS-Direct-Ozone-in-Troposphere) method that uses TOMS radiances and a modified lookup table based on actual profiles during high ozone pollution periods, new maps were prepared and found to compare better to soundings over Lusaka, Zambia (15.5 S, 28 E), Nairobi and several African cities where MOZAIC aircraft operated in September 2000. The TDOT technique and comparisons are described in detail.

  15. Performance Evaluation of Blind Tropospheric Delay correction ...

    African Journals Online (AJOL)

    This report represents an appraisal of the performance of the GPT2w and UNB3M models with accurate International GNSS Service (IGS)- tropospheric estimations for fifteen IGS stations over a period of 1 year on the Africa continent. Both models perform significantly better at low latitudes than higher latitudes. There was ...

  16. Tropospheric ozone. Formation, properties, effects. Expert opinion

    International Nuclear Information System (INIS)

    Elstner, E.F.

    1996-01-01

    The formation and dispersion of tropospheric ozone are discussed only marginally in this expert opinion; the key interest is in the effects of ground level ozone on plants, animals, and humans. The expert opinion is based on an analysis of the available scientific publications. (orig./MG) [de

  17. TROPOSPHERIC AEROSOL PROGRAM, PROGRAM PLAN, MARCH 2001

    Energy Technology Data Exchange (ETDEWEB)

    SCHWARTZ,S.E.; LUNN,P.

    2001-03-01

    The goal of Tropospheric Aerosol Program (TAP) will be to develop the fundamental scientific understanding required to construct tools for simulating the life cycle of tropospheric aerosols--the processes controlling their mass loading, composition, and microphysical properties, all as a function of time, location, and altitude. The TAP approach to achieving this goal will be by conducting closely linked field, modeling, laboratory, and theoretical studies focused on the processes controlling formation, growth, transport, and deposition of tropospheric aerosols. This understanding will be represented in models suitable for describing these processes on a variety of geographical scales; evaluation of these models will be a key component of TAP field activities. In carrying out these tasks TAP will work closely with other programs in DOE and in other Federal and state agencies, and with the private sector. A forum to directly work with our counterparts in industry to ensure that the results of this research are translated into products that are useful to that community will be provided by NARSTO (formerly the North American Research Strategy on Tropospheric Ozone), a public/private partnership, whose membership spans government, the utilities, industry, and university researchers in Mexico, the US, and Canada.

  18. Spherical zonal components of cosmic ray between Forbush decreases

    International Nuclear Information System (INIS)

    Takahashi, Hachiro; Yahagi, Naohiro; Nagashima, Kazuo.

    1974-01-01

    Two examples are added to the previous report on the zonal harmonic components of cosmic ray in the space between planets by the three dimensional analysis of anisotropy of cosmic ray. Remarkable Forbush decreases occurred in region I during the period from March 20th to April 11th, 1966 and in region II during the period from August 29th to September 11th, 1966. The data used for analysis are the neutron components that have been informed from cosmic ray observation stations in the world. Power type and power exponential type differential rigidity spectra G(P) were used to find isotropic components. The change of the isotropic component a 0 0 was similar to the change of the neutron intensity in Deep River. The southnorth anisotropic phenomenon of cosmic ray intensity was recognized. The anisotropy in the opposite direction to the southnorth anisotropic phenomenon reported by Nagashima et al. was recognized markedly during the period from March 26th to 30th. These tendencies were checked by comparing with the data from the cosmic ray observation stations located near both poles of the earth. McMurdo and Mawson near the south pole, and Thule and Alert near the north pole were selected. The results of analysis were confirmed with these data. Further, the results of the previous report were checked by using the data from the stations near both poles, namely Thule, Resolute Bay, and Mawson. The good coincidence was confirmed on the anisotropic components. (Iwakiri, K.)

  19. Zonal-flow dynamics from a phase-space perspective

    Science.gov (United States)

    Ruiz, D. E.; Parker, J. B.; Shi, E. L.; Dodin, I. Y.

    2017-10-01

    The wave kinetic equation (WKE) describing drift-wave (DW) turbulence is widely used in the studies of zonal flows (ZFs) emerging from DW turbulence. However, this formulation neglects the exchange of enstrophy between DWs and ZFs and also ignores effects beyond the geometrical-optics (GO) limit. Here we present a new theory that captures both of these effects, while still treating DW quanta (``driftons'') as particles in phase space. In this theory, the drifton dynamics is described by an equation of the Wigner-Moyal type, which is analogous to the phase-space formulation of quantum mechanics. The ``Hamiltonian'' and the ``dissipative'' parts of the DW-ZF interactions are clearly identified. Moreover, this theory can be interpreted as a phase-space representation of the second-order cumulant expansion (CE2). In the GO limit, this formulation features additional terms missing in the traditional WKE that ensure conservation of the total enstrophy of the system, in addition to the total energy, which is the only conserved invariant in previous theories based on the traditional WKE. Numerical simulations are presented to illustrate the importance of these additional terms. Supported by the U.S. DOE through Contract Nos. DE-AC02-09CH11466 and DE-AC52-07NA27344, by the NNSA SSAA Program through DOE Research Grant No. DE-NA0002948, and by the U.S. DOD NDSEG Fellowship through Contract No. 32-CFR-168a.

  20. Characteristics of intercontinental transport of tropospheric ozone from Africa to Asia

    Science.gov (United States)

    Han, Han; Liu, Jane; Yuan, Huiling; Zhuang, Bingliang; Zhu, Ye; Wu, Yue; Yan, Yuhan; Ding, Aijun

    2018-03-01

    In this study, we characterize the transport of ozone from Africa to Asia through the analysis of the simulations of a global chemical transport model, GEOS-Chem, from 1987 to 2006. The receptor region Asia is defined within 5-60° N and 60-145° E, while the source region Africa is within 35° S-15° N and 20° W-55° E and within 15-35° N and 20° W-30° E. The ozone generated in the African troposphere from both natural and anthropogenic sources is tracked through tagged ozone simulation. Combining this with analysis of trajectory simulations using the Hybrid Single-Particle Lagrangian Integrated Trajectory (HYSPLIT) model, we find that the upper branch of the Hadley cell connects with the subtropical westerlies in the Northern Hemisphere (NH) to form a primary transport pathway from Africa to Asia in the middle and upper troposphere throughout the year. The Somali jet that runs from eastern Africa near the equator to the Indian subcontinent in the lower troposphere is the second pathway that appears only in NH summer. The influence of African ozone mainly appears over Asia south of 40° N. The influence shows strong seasonality, varying with latitude, longitude, and altitude. In the Asian upper troposphere, imported African ozone is largest from March to May around 30° N (12-16 ppbv) and lowest during July-October around 10° N ( ˜ 2 ppbv). In the Asian middle and lower troposphere, imported African ozone peaks in NH winter between 20 and 25° N. Over 5-40° N, the mean fractional contribution of imported African ozone to the overall ozone concentrations in Asia is largest during NH winter in the middle troposphere ( ˜ 18 %) and lowest in NH summer throughout the tropospheric column ( ˜ 6 %). This seasonality mainly results from the collective effects of the ozone precursor emissions in Africa and meteorology and chemistry in Africa, in Asia and along the transport pathways. The seasonal swing of the Hadley circulation and subtropical westerlies along the

  1. Wind Diffusivity Current, METOP ASCAT, 0.25 degrees, Global, Near Real Time, Zonal

    Data.gov (United States)

    National Oceanic and Atmospheric Administration, Department of Commerce — NOAA CoastWatch distributes near real time Ekman current (in zonal, meridional, and modulus sets) and Ekman upwelling data. This data begins with wind velocity...

  2. HIRDLS/Aura Level 3 Extinction at 12.1 Microns Zonal Fourier Coefficients V007

    Data.gov (United States)

    National Aeronautics and Space Administration — The "HIRDLS/Aura Level 3 Extinction at 12.1 Microns Zonal Fourier Coefficients" version 7 data product (H3ZFC12MEXT) contains the entire mission (~3 years) of HIRDLS...

  3. Wind Stress, METOP ASCAT, 0.25 degrees, Global, Near Real Time, Zonal

    Data.gov (United States)

    National Oceanic and Atmospheric Administration, Department of Commerce — NOAA CoastWatch distributes near real time wind stress data in zonal, meridional, modulus, and wind stress curl sets. This data begins with wind velocity...

  4. Wind Stress, QuikSCAT SeaWinds, 0.25 degrees, Global, Science Quality, Zonal

    Data.gov (United States)

    National Oceanic and Atmospheric Administration, Department of Commerce — NOAA CoastWatch distributes science quality wind stress data in zonal, meridional, modulus, and wind stress curl sets. This data begins with wind velocity...

  5. Currents, HF Radio-derived, Monterey Bay, Normal Model, Zonal, EXPERIMENTAL

    Data.gov (United States)

    National Oceanic and Atmospheric Administration, Department of Commerce — The data is the zonal component of ocean surface currents derived from High Frequency Radio-derived measurements, with missing values filled in by a normal model....

  6. Currents, HF Radio-derived, Monterey Bay, 25 hr, Zonal, EXPERIMENTAL

    Data.gov (United States)

    National Oceanic and Atmospheric Administration, Department of Commerce — The data is the 25 hour running average of the zonal component of ocean surface currents derived from High Frequency Radio-derived measurements. THIS IS AN...

  7. TOMS/EP UV Reflectivity Daily and Monthly Zonal Means V008

    Data.gov (United States)

    National Aeronautics and Space Administration — This data product contains TOMS/EP UV Reflectivity Daily and Monthly Zonal Means Version 8 data in ASCII format. (The shortname for this Level-3 Earth Probe TOMS...

  8. Currents, HF Radio-derived, Ano Nuevo, 25 hr, Zonal, EXPERIMENTAL

    Data.gov (United States)

    National Oceanic and Atmospheric Administration, Department of Commerce — The data is the 25 hour running average of the zonal component of ocean surface currents derived from High Frequency Radio-derived measurements. THIS IS AN...

  9. Generation of zonal flow in the Earth's dissipative ionospheric F-layer

    International Nuclear Information System (INIS)

    Kaladze, T.D.; Shad, M.; Tsamalashvili, L.V.

    2011-01-01

    Generation of zonal flow in the Earth's dissipative ionospheric F-layer is considered. Dissipation arises due to Pedersen conductivity acting as an inductive (magnetic) inhibition. It is shown that in contrast to previous investigations the zonal flow growth rate does not depend on small wave vector component of zonal flow mode, needs no instability condition and the spectral energy transferring (inverse cascade) process unconditionally takes place. -- Highlights: → Generation of zonal flow in the Earth's dissipative ionospheric F-layer is considered. → Dissipation arises due to Pedersen conductivity acting as inductive (magnetic) inhibition. → It is shown that such generation doesn't need any instability condition. → Energy transferring (inverse cascade) process takes place even for the small values of pumping intensity.

  10. Nonlinear entropy transfer in ETG-TEM turbulence via TEM driven zonal flows

    International Nuclear Information System (INIS)

    Asahi, Yuuichi; Tsutsui, Hiroaki; Tsuji-Iio, Shunji; Ishizawa, Akihiro; Sugama, Hideo; Watanabe, Tomohiko

    2015-01-01

    Nonlinear interplay of the electron temperature gradient (ETG) modes and the trapped electron modes (TEMs) was investigated by means of gyrokinetic simulation. Focusing on the situation where both TEMs and ETG modes are linearly unstable, the effects of TEM-driven zonal flows on ETG turbulence were examined by means of entropy transfer analysis. In a statistically steady turbulence where the TEM driven zonal flows are dominant, it turned out that the zonal flows meditate the entropy transfer of the ETG modes from the low to high radial wavenumber regions. The successive entropy transfer broadens the potential fluctuation spectrum in the radial wavenumber direction. In contrast, in the situation where ETG modes are unstable but TEMs are stable, the pure ETG turbulence does not produce strong zonal flows, leading to a rather narrow spectrum in the radial wavenumber space and a higher transport level. (author)

  11. Atmospheric statistical dynamic models. Model performance: the Lawrence Livermore Laboratoy Zonal Atmospheric Model

    International Nuclear Information System (INIS)

    Potter, G.L.; Ellsaesser, H.W.; MacCracken, M.C.; Luther, F.M.

    1978-06-01

    Results from the zonal model indicate quite reasonable agreement with observation in terms of the parameters and processes that influence the radiation and energy balance calculations. The model produces zonal statistics similar to those from general circulation models, and has also been shown to produce similar responses in sensitivity studies. Further studies of model performance are planned, including: comparison with July data; comparison of temperature and moisture transport and wind fields for winter and summer months; and a tabulation of atmospheric energetics. Based on these preliminary performance studies, however, it appears that the zonal model can be used in conjunction with more complex models to help unravel the problems of understanding the processes governing present climate and climate change. As can be seen in the subsequent paper on model sensitivity studies, in addition to reduced cost of computation, the zonal model facilitates analysis of feedback mechanisms and simplifies analysis of the interactions between processes

  12. Currents, HF Radio-derived, SF Bay, 25 hr, Zonal, EXPERIMENTAL

    Data.gov (United States)

    National Oceanic and Atmospheric Administration, Department of Commerce — The data is the 25 hour running average of the zonal component of ocean surface currents derived from High Frequency Radio-derived measurements. THIS IS AN...

  13. Zonal Flows Driven by Small-Scale Drift-Alfven Modes

    International Nuclear Information System (INIS)

    Li Dehui; Zhou Deng

    2011-01-01

    Generation of zonal flows by small-scale drift-Alfven modes is investigated by adopting the approach of parametric instability with the electron polarization drift included. The zonal mode can be excited by primary modes propagating at both electron and ion diamagnetic drift directions in contrast to the assertion in previous studies that only primary modes propagating in the ion diamagnetic drift directions can drive zonal instabilities. Generally, the growth rate of the driven zonal mode is in the same order as that in previous study. However, different from the previous work, the growth rate is no longer proportional to the difference between the diamagnetic drift frequencies of electrons and ions. (magnetically confined plasma)

  14. Regulation of electron temperature gradient turbulence by zonal flows driven by trapped electron modes

    Science.gov (United States)

    Asahi, Y.; Ishizawa, A.; Watanabe, T.-H.; Tsutsui, H.; Tsuji-Iio, S.

    2014-05-01

    Turbulent transport caused by electron temperature gradient (ETG) modes was investigated by means of gyrokinetic simulations. It was found that the ETG turbulence can be regulated by meso-scale zonal flows driven by trapped electron modes (TEMs), which are excited with much smaller growth rates than those of ETG modes. The zonal flows of which radial wavelengths are in between the ion and the electron banana widths are not shielded by trapped ions nor electrons, and hence they are effectively driven by the TEMs. It was also shown that an E × B shearing rate of the TEM-driven zonal flows is larger than or comparable to the growth rates of long-wavelength ETG modes and TEMs, which make a main contribution to the turbulent transport before excitation of the zonal flows.

  15. Currents, HF Radio-derived, SF Bay, 1 hr, Zonal, EXPERIMENTAL

    Data.gov (United States)

    National Oceanic and Atmospheric Administration, Department of Commerce — The data is the 1 hour average of the zonal component of ocean surface currents derived from High Frequency Radio-derived measurements. THIS IS AN EXPERIMENTAL...

  16. Currents, HF Radio-derived, Bodega Bay, 1 hr, Zonal, EXPERIMENTAL

    Data.gov (United States)

    National Oceanic and Atmospheric Administration, Department of Commerce — The data is the 1 hour average of the zonal component of ocean surface currents derived from High Frequency Radio-derived measurements. THIS IS AN EXPERIMENTAL...

  17. The temperature signature of an IMF-driven change to the global atmospheric electric circuit (GEC) in the Antarctic troposphere

    Science.gov (United States)

    Freeman, Mervyn; Lam, Mai Mai; Chisham, Gareth

    2017-04-01

    We use National Centers for Environmental Prediction (NCEP)/National Center for Atmospheric Research (NCAR) reanalysis data to show that Antarctic surface air temperature anomalies result from differences in the daily-mean duskward component,By, of the interplanetary magnetic field (IMF). We find the anomalies have strong geographical and seasonal variations. Regional anomalies are evident poleward of 60˚ S and are of diminishing representative peak amplitude from autumn (3.2˚ C) to winter (2.4˚ C) to spring (1.6˚ C) to summer (0.9˚ C). We demonstrate that anomalies of statistically-significant amplitude are due to geostrophic wind anomalies, resulting from the same By changes, moving air across large meridional gradients in zonal mean air temperature between 60 and 80˚ S. Additionally, we find that the mean tropospheric temperature anomaly for geographical latitudes ≤ -70˚ peaks at about 0.7 K and is statistically significant at the 1 - 5% level between air pressures of 1000 and 500 hPa (i.e., ˜0.1 to 5.6 km altitude above sea level) and for time lags with respect to the IMF of up to 7 days. The signature propagates vertically between air pressure p ≥ 850 hPa (≤ 1.5 km) and p = 500 hPa (˜5.6 km). The characteristics of prompt response and vertical propagation within the troposphere have previously been seen in the correlation between the IMF and high-latitude air pressure anomalies, known as the Mansurov effect, at higher statistical significances (1%). We conclude that we have identified the temperature signature of the Mansurov effect in the Antarctic troposphere. Since these tropospheric anomalies have been associated with By-driven anomalies in the electric potential of the ionosphere, we further conclude that they are caused by IMF-induced changes to the global atmospheric electric circuit (GEC). Our results support the view that variations in the ionospheric potential act on the troposphere via the action of resulting variations in the

  18. Ground-based remote sensing of tropospheric water vapour isotopologues within the project MUSICA

    Directory of Open Access Journals (Sweden)

    M. Schneider

    2012-12-01

    Full Text Available Within the project MUSICA (MUlti-platform remote Sensing of Isotopologues for investigating the Cycle of Atmospheric water, long-term tropospheric water vapour isotopologue data records are provided for ten globally distributed ground-based mid-infrared remote sensing stations of the NDACC (Network for the Detection of Atmospheric Composition Change. We present a new method allowing for an extensive and straightforward characterisation of the complex nature of such isotopologue remote sensing datasets. We demonstrate that the MUSICA humidity profiles are representative for most of the troposphere with a vertical resolution ranging from about 2 km (in the lower troposphere to 8 km (in the upper troposphere and with an estimated precision of better than 10%. We find that the sensitivity with respect to the isotopologue composition is limited to the lower and middle troposphere, whereby we estimate a precision of about 30‰ for the ratio between the two isotopologues HD16O and H216O. The measurement noise, the applied atmospheric temperature profiles, the uncertainty in the spectral baseline, and the cross-dependence on humidity are the leading error sources. We introduce an a posteriori correction method of the cross-dependence on humidity, and we recommend applying it to isotopologue ratio remote sensing datasets in general. In addition, we present mid-infrared CO2 retrievals and use them for demonstrating the MUSICA network-wide data consistency. In order to indicate the potential of long-term isotopologue remote sensing data if provided with a well-documented quality, we present a climatology and compare it to simulations of an isotope incorporated AGCM (Atmospheric General Circulation Model. We identify differences in the multi-year mean and seasonal cycles that significantly exceed the estimated errors, thereby indicating deficits in the modeled atmospheric water cycle.

  19. Ground-based remote sensing of tropospheric water vapour isotopologues within the project MUSICA

    Science.gov (United States)

    Schneider, M.; Barthlott, S.; Hase, F.; González, Y.; Yoshimura, K.; García, O. E.; Sepúlveda, E.; Gomez-Pelaez, A.; Gisi, M.; Kohlhepp, R.; Dohe, S.; Blumenstock, T.; Wiegele, A.; Christner, E.; Strong, K.; Weaver, D.; Palm, M.; Deutscher, N. M.; Warneke, T.; Notholt, J.; Lejeune, B.; Demoulin, P.; Jones, N.; Griffith, D. W. T.; Smale, D.; Robinson, J.

    2012-12-01

    Within the project MUSICA (MUlti-platform remote Sensing of Isotopologues for investigating the Cycle of Atmospheric water), long-term tropospheric water vapour isotopologue data records are provided for ten globally distributed ground-based mid-infrared remote sensing stations of the NDACC (Network for the Detection of Atmospheric Composition Change). We present a new method allowing for an extensive and straightforward characterisation of the complex nature of such isotopologue remote sensing datasets. We demonstrate that the MUSICA humidity profiles are representative for most of the troposphere with a vertical resolution ranging from about 2 km (in the lower troposphere) to 8 km (in the upper troposphere) and with an estimated precision of better than 10%. We find that the sensitivity with respect to the isotopologue composition is limited to the lower and middle troposphere, whereby we estimate a precision of about 30‰ for the ratio between the two isotopologues HD16O and H216O. The measurement noise, the applied atmospheric temperature profiles, the uncertainty in the spectral baseline, and the cross-dependence on humidity are the leading error sources. We introduce an a posteriori correction method of the cross-dependence on humidity, and we recommend applying it to isotopologue ratio remote sensing datasets in general. In addition, we present mid-infrared CO2 retrievals and use them for demonstrating the MUSICA network-wide data consistency. In order to indicate the potential of long-term isotopologue remote sensing data if provided with a well-documented quality, we present a climatology and compare it to simulations of an isotope incorporated AGCM (Atmospheric General Circulation Model). We identify differences in the multi-year mean and seasonal cycles that significantly exceed the estimated errors, thereby indicating deficits in the modeled atmospheric water cycle.

  20. Oxygenated Organic Chemicals in the Pacific Troposphere: Distribution, Sources and Chemistry

    Science.gov (United States)

    Singh, Hanwant B.; Salas, L.; Chatfield, R.; Czech, E.; Fried, A.; Evans, M.; Jacob, D. J.; Blake, D.; Heikes, B.; Talbot, R.

    2003-01-01

    Airborne measurements of a large number of oxygenated organic chemicals (Oxorgs) were carried out in the Pacific troposphere (0.1-12 km) in the Spring of 2001 (Feb. 24-April 10). Specifically these measuremen ts included acetone, methylethyl ketone (MEK), methanol, ethanol, ace taldehyde, propionaldehyde, PANS, and organic nitrates. Complementary measurements of formaldehyde, organic peroxides, and tracers were al so available. Ox-orgs were abundant in the clean troposphere and were greatly enhanced in the outflow regions from Asia. Their mixing ratios were typically highest in the lower troposphere and declined toward s the upper troposphere and the lowermost stratosphere. Their total a bundance (Ox-orgs) significantly exceeded that of NMHC (C2-C8 NMHC). A comparison of these data with observations collected some seven yea rs earlier (Feb.-March, 1994), did not reveal any significant changes . Throughout the troposphere mixing ratios of Ox-orgs were strongly c orrelated with each other as well as with tracers of fossil and bioma sshiof'uel combustion. Analysis of the relative enhancement of selected Oxorgs with respect to CH3Cl and CO in twelve sampled plumes, origi nating from fires, is used to assess their primary and secondary sour ces from biomass combustion. The composition of these plumes also ind icates a large shift of reactive nitrogen into the PAN reservoir ther eby limiting ozone formation. The Harvard 3-D photochemical model, th at uses state of the art chemistry and source information, is used to compare simulated and observed mixing ratios of selected species. A 1 -D model is used to explore the chemistry of aldehydes. These results will be presented.

  1. The Role of Reversed Equatorial Zonal Transport in Terminating an ENSO Event

    Science.gov (United States)

    Chen, H. C.; Hu, Z. Z.; Huang, B.; Sui, C. H.

    2016-02-01

    In this study, we demonstrate that a sudden reversal of anomalous equatorial zonal current at the peaking ENSO phase triggers the rapid termination of an ENSO event. Throughout an ENSO cycle, the anomalous equatorial zonal current is strongly controlled by the concavity of the anomalous thermocline meridional structure near the equator. During the ENSO developing phase, the anomalous zonal current in the central and eastern Pacific generally enhances the ENSO growth through its zonal SST advection. In the mature phase of ENSO, however, the equatorial thermocline depth anomalies are reflected in the eastern Pacific and slowly propagate westward off the equator in both hemispheres. As a result, the concavity of the thermocline anomalies near the equator is reversed, i.e., the off-equatorial thermocline depth anomalies become higher than that on the equator for El Niño events and lower for La Niño events. This meridional change of thermocline structure reverses zonal transport rapidly in the central-to-eastern equatorial Pacific, which weakens the ENSO SST anomalies by reversed advection. More importantly, the reversed zonal mass transport weakens the existing zonal tilting of equatorial thermocline and suppresses the thermocline feedback. Both processes are concentrated in the eastern equatorial Pacific and can be effective on subseasonal time scales. These current reversal effects are built-in to the ENSO peak phase and independent of the zonal wind effect on thermocline slope. It functions as an oceanic control on ENSO evolution during both El Niño and La Niña events.

  2. Impact of uncertainties in inorganic chemical rate constants on tropospheric composition and ozone radiative forcing

    Directory of Open Access Journals (Sweden)

    B. Newsome

    2017-12-01

    regions such as the tropics, poles and upper troposphere are most uncertain. This chemical uncertainty is sufficiently large to suggest that rate constant uncertainty should be considered alongside other processes when model results disagree with measurement. Calculations for the pre-industrial simulation allow a tropospheric ozone radiative forcing to be calculated of 0.412 ± 0.062 W m−2. This uncertainty (13 % is comparable to the inter-model spread in ozone radiative forcing found in previous model–model intercomparison studies where the rate constants used in the models are all identical or very similar. Thus, the uncertainty of tropospheric ozone radiative forcing should expanded to include this additional source of uncertainty. These rate constant uncertainties are significant and suggest that refinement of supposedly well-known chemical rate constants should be considered alongside other improvements to enhance our understanding of atmospheric processes.

  3. Experimental particle formation rates spanning tropospheric sulfuric acid and ammonia abundances, ion production rates, and temperatures

    CERN Document Server

    Kürten, Andreas; Almeida, Joao; Kupiainen-Määttä, Oona; Dunne, Eimear M.; Duplissy, Jonathan; Williamson, Christina; Barmet, Peter; Breitenlechner, Martin; Dommen, Josef; Donahue, Neil M.; Flagan, Richard C.; Franchin, Alessandro; Gordon, Hamish; Hakala, Jani; Hansel, Armin; Heinritzi, Martin; Ickes, Luisa; Jokinen, Tuija; Kangasluoma, Juha; Kim, Jaeseok; Kirkby, Jasper; Kupc, Agnieszka; Lehtipalo, Katrianne; Leiminger, Markus; Makhmutov, Vladimir; Onnela, Antti; Ortega, Ismael K.; Petäjä, Tuukka; Praplan, Arnaud P.; Riccobono, Francesco; Rissanen, Matti P.; Rondo, Linda; Schnitzhofer, Ralf; Schobesberger, Siegfried; Smith, James N.; Steiner, Gerhard; Stozhkov, Yuri; Tomé, António; Tröstl, Jasmin; Tsagkogeorgas, Georgios; Wagner, Paul E.; Wimmer, Daniela; Ye, Penglin; Baltensperger, Urs; Carslaw, Ken; Kulmala, Markku; Curtius, Joachim

    2016-01-01

    Binary nucleation of sulfuric acid and water as well as ternary nucleation involving ammonia arethought to be the dominant processes responsible for new particle formation (NPF) in the cold temperaturesof the middle and upper troposphere. Ions are also thought to be important for particle nucleation inthese regions. However, global models presently lack experimentally measured NPF rates under controlledlaboratory conditions and so at present must rely on theoretical or empirical parameterizations. Here withdata obtained in the European Organization for Nuclear Research CLOUD (Cosmics Leaving OUtdoor Droplets)chamber, we present the first experimental survey of NPF rates spanning free tropospheric conditions. Theconditions during nucleation cover a temperature range from 208 to 298 K, sulfuric acid concentrationsbet ween 5 × 105and 1 × 109cm3, and ammonia mixing ratios from zero added ammonia, i.e., nominally purebinary, to a maximum of ~1400 parts per trillion by volume (pptv). We performed nucleation s...

  4. Direct electron crystallographic determination of zeolite zonal structures

    International Nuclear Information System (INIS)

    Dorset, Douglas L.; Gilmore, Christopher J.; Jorda, Jose Luis; Nicolopoulos, Stavros

    2007-01-01

    The prospect for improving the success of ab initio zeolite structure investigations with electron diffraction data is evaluated. First of all, the quality of intensities obtained by precession electron diffraction at small hollow cone illumination angles is evaluated for seven representative materials: ITQ-1, ITQ-7, ITQ-29, ZSM-5, ZSM-10, mordenite, and MCM-68. It is clear that, for most examples, an appreciable fraction of a secondary scattering perturbation is removed by precession at small angles. In one case, ZSM-10, it can also be argued that precession diffraction produces a dramatically improved 'kinematical' data set. There seems to no real support for application of a Lorentz correction to these data and there is no reason to expect for any of these samples that a two-beam dynamical scattering relationship between structure factor amplitude and observed intensity should be valid. Removal of secondary scattering by the precession mode appears to facilitate ab initio structure analysis. Most zeolite structures investigated could be solved by maximum entropy and likelihood phasing via error-correcting codes when precession data were used. Examples include the projected structure of mordenite that could not be determined from selected area data alone. One anomaly is the case of ZSM-5, where the best structure determination in projection is made from selected area diffraction data. In a control study, the zonal structure of SSZ-48 could be determined from selected area diffraction data by either maximum entropy and likelihood or traditional direct methods. While the maximum entropy and likelihood approach enjoys some advantages over traditional direct methods (non-dependence on predicted phase invariant sums), some effort must be made to improve the figures of merit used to identify potential structure solutions

  5. Model test of anchoring effect on zonal disintegration in deep surrounding rock masses.

    Science.gov (United States)

    Chen, Xu-Guang; Zhang, Qiang-Yong; Wang, Yuan; Liu, De-Jun; Zhang, Ning

    2013-01-01

    The deep rock masses show a different mechanical behavior compared with the shallow rock masses. They are classified into alternating fractured and intact zones during the excavation, which is known as zonal disintegration. Such phenomenon is a great disaster and will induce the different excavation and anchoring methodology. In this study, a 3D geomechanics model test was conducted to research the anchoring effect of zonal disintegration. The model was constructed with anchoring in a half and nonanchoring in the other half, to compare with each other. The optical extensometer and optical sensor were adopted to measure the displacement and strain changing law in the model test. The displacement laws of the deep surrounding rocks were obtained and found to be nonmonotonic versus the distance to the periphery. Zonal disintegration occurs in the area without anchoring and did not occur in the model under anchoring condition. By contrasting the phenomenon, the anchor effect of restraining zonal disintegration was revealed. And the formation condition of zonal disintegration was decided. In the procedure of tunnel excavation, the anchor strain was found to be alternation in tension and compression. It indicates that anchor will show the nonmonotonic law during suppressing the zonal disintegration.

  6. Changes in Jupiter's Zonal Wind Profile Preceding and During the Juno Mission

    Science.gov (United States)

    Tollefson, Joshua; Wong, Michael H.; de Pater, Imke; Simon, Amy A.; Orton, Glenn S.; Rogers, John H.; Atreya, Sushil K.; Cosentino, Richard G.; Januszewski, William; Morales-Juberias, Raul; hide

    2017-01-01

    We present five epochs of WFC3 HST Jupiter observations taken between 2009-2016 and extract global zonal wind profiles for each epoch. Jupiter's zonal wind field is globally stable throughout these years, but significant variations in certain latitude regions persist. We find that the largest uncertainties in the wind field are due to vortices or hot-spots, and show residual maps which identify the strongest vortex flows. The strongest year-to-year variation in the zonal wind profiles is the 24 deg N jet peak. Numerous plume outbreaks have been observed in the Northern Temperate Belt and are associated with decreases in the zonal velocity and brightness. We show that the 24 deg N jet peak velocity and brightness decreased in 2012 and again in late 2016, following outbreaks during these years. Our February 2016 zonal wind profile was the last highly spatially resolved measurement prior to Juno s first science observations. The final 2016 data were taken in conjunction with Juno's perijove 3 pass on 11 December 2016, and show the zonal wind profile following the plume outbreak at 24 deg N in October 2016.

  7. Model Test of Anchoring Effect on Zonal Disintegration in Deep Surrounding Rock Masses

    Directory of Open Access Journals (Sweden)

    Xu-Guang Chen

    2013-01-01

    Full Text Available The deep rock masses show a different mechanical behavior compared with the shallow rock masses. They are classified into alternating fractured and intact zones during the excavation, which is known as zonal disintegration. Such phenomenon is a great disaster and will induce the different excavation and anchoring methodology. In this study, a 3D geomechanics model test was conducted to research the anchoring effect of zonal disintegration. The model was constructed with anchoring in a half and nonanchoring in the other half, to compare with each other. The optical extensometer and optical sensor were adopted to measure the displacement and strain changing law in the model test. The displacement laws of the deep surrounding rocks were obtained and found to be nonmonotonic versus the distance to the periphery. Zonal disintegration occurs in the area without anchoring and did not occur in the model under anchoring condition. By contrasting the phenomenon, the anchor effect of restraining zonal disintegration was revealed. And the formation condition of zonal disintegration was decided. In the procedure of tunnel excavation, the anchor strain was found to be alternation in tension and compression. It indicates that anchor will show the nonmonotonic law during suppressing the zonal disintegration.

  8. Effect of mean flow on the interaction between turbulence and zonal flow

    International Nuclear Information System (INIS)

    Uzawa, Ken; Kishimoto, Yasuaki; Li Jiquan

    2006-01-01

    The effects of an external mean flow on the generation of zonal flow in drift wave turbulence are theoretically studied in terms of a modulational instability analysis. A dispersion relation for the zonal flow instability having complex frequency ω q =Ω q +iγ q is derived, which depends on the external mean flow's amplitude |φ f | and radial wave number k f . As an example, we chose an ion temperature gradient (ITG) turbulence-driven zonal flow as the mean flow acting on an electron temperature gradient (ETG) turbulence-zonal flow system. The growth rate of the zonal flow γ q is found to be suppressed, showing a relation γ q =γ q0 (1 - α|φ f | 2 k f 2 ), where γ q0 is the growth rate in the absence of mean flow and α is a positive numerical constant. This formula is applicable to a strong shearing regime where the zonal flow instability is stabilized at α|φ f 2 |k f 2 ≅ 1. Meanwhile, the suppression is accompanied by an increase of the real frequency |Ω q |. The underlying physical mechanism of the suppression is discussed. (author)

  9. Interpretation of TOMS Observations of Tropical Tropospheric Ozone with a Global Model and In Situ Observations

    Science.gov (United States)

    Martin, Randall V.; Jacob, Daniel J.; Logan, Jennifer A.; Bey, Isabelle; Yantosca, Robert M.; Staudt, Amanda C.; Fiore, Arlene M.; Duncan, Bryan N.; Liu, Hongyu; Ginoux, Paul

    2004-01-01

    We interpret the distribution of tropical tropospheric ozone columns (TTOCs) from the Total Ozone Mapping Spectrometer (TOMS) by using a global three-dimensional model of tropospheric chemistry (GEOS-CHEM) and additional information from in situ observations. The GEOS-CHEM TTOCs capture 44% of the variance of monthly mean TOMS TTOCs from the convective cloud differential method (CCD) with no global bias. Major discrepancies are found over northern Africa and south Asia where the TOMS TTOCs do not capture the seasonal enhancements from biomass burning found in the model and in aircraft observations. A characteristic feature of these northern topical enhancements, in contrast to southern tropical enhancements, is that they are driven by the lower troposphere where the sensitivity of TOMS is poor due to Rayleigh scattering. We develop an efficiency correction to the TOMS retrieval algorithm that accounts for the variability of ozone in the lower troposphere. This efficiency correction increases TTOC's over biomass burning regions by 3-5 Dobson units (DU) and decreases them by 2-5 DU over oceanic regions, improving the agreement between CCD TTOCs and in situ observations. Applying the correction to CCD TTOCs reduces by approximately DU the magnitude of the "tropical Atlantic paradox" [Thompson et al, 2000], i.e. the presence of a TTOC enhancement over the southern tropical Atlantic during the northern African biomass burning season in December-February. We reproduce the remainder of the paradox in the model and explain it by the combination of upper tropospheric ozone production from lightning NOx, peristent subsidence over the southern tropical Atlantic as part of the Walker circulation, and cross-equatorial transport of upper tropospheric ozone from northern midlatitudes in the African "westerly duct." These processes in the model can also account for the observed 13-17 DU persistent wave-1 pattern in TTOCs with a maximum above the tropical Atlantic and a minimum

  10. Integrating chemistry into 3D climate models: Detailed kinetics in the troposphere and stratosphere of a global climate model

    Energy Technology Data Exchange (ETDEWEB)

    Kao, C.Y.J.; Elliott, S. [Los Alamos National Lab., NM (United States). Earth and Environmental Sciences Div.; Turco, R.P.; Zhao, X. [Univ. of California, Los Angeles, CA (United States)

    1997-11-01

    This is the final report of a three-year, Laboratory Directed Research and Development (LDRD) project at Los Alamos National Laboratory (LANL). The motivation for the project is to create the first complete, three-dimensional climate model that enfolds atmospheric photochemistry. The LANL chemical global climate model (GCM) not only distributes the trace greenhouse gases and modifies their concentrations within the detailed photochemical web, but also permits them to influence the radiation field and so force their own transport. Both atmospheric chemistry and fluid dynamics are nonlinear and zonally asymmetric phenomena. They can only be adequately modeled in three dimensions on the global grid. The kinetics-augmented GCM is the only program within the atmospheric community capable of investigating interaction involving chemistry and transport. The authors have conducted case studies of timely three-dimensional chemistry issues. Examples include ozone production from biomass burning plumes, kinetic feedbacks in zonally asymmetric transport phenomena with month- to year-long time scales, and volcano sulfate aerosols with respect to their potential effects on tropospheric ozone depletion.

  11. Tropospheric Delay from VLBI and GNSS Measurements

    Science.gov (United States)

    Gubanov, V. S.

    2018-02-01

    Using an updated version of the QUASAR software package developed at the Institute of Applied Astronomy of the Russian Academy of Sciences, we have processed the VLBI observations within the international CONT14 program (May 6-20, 2014), in which a global network of 17 stations was involved (a total of 250 000 observations). The package update concerned the optimization of data structure and the refinement of stochastic models for the random variations in wet tropospheric delay and atomic clock difference. The main goal of this paper is to compare the VLBI determinations of the tropospheric delay with its independent determinations using global navigation satellite systems (GNSS). We show that both these determinations agree well between themselves only in the case of a global analysis of the VLBI observations, where the VLBI station coordinates are also refined, along with the tropospheric delay and the clock synchronization and Earth orientation parameters. If, alternatively, the station coordinates are insufficiently accurate and are not refined from VLBI observations, then it is appropriate not to determine the tropospheric delay from these observations, but to take it from the publicly accessible independent GNSS data. However, this requires that the VLBI and GNSS techniques operate simultaneously at a common observing site. We have established the shortcomings of the universally accepted method of stabilizing the global solution associated with the absence of a criterion for choosing reference stations and radio sources. Two ways of their elimination are proposed: (i) introducing a coordinated list of weight factors for the errors in the coordinates of such stations and sources into the stabilization algorithm and (ii) adopting a coordinated list of stations and sources the refinement of whose coordinates is not required at all for a certain time.

  12. Radon concentration inversions in the troposphere

    International Nuclear Information System (INIS)

    Pereira, E.B.

    1987-07-01

    Vertical concentrations of radon in the lower troposphere were obtained in Southern Brazil up to 7Km high and have shown unexpected inverted profiles. The presence of low pressure center systems southwest to the flight path suggested that inversions might have been originated by a vertical transport mechanism based on the large scale circulation of developing synoptic systems. A simple friction-driven circulation model was contructed and the transport equation was solved. (author) [pt

  13. Tropospheric radiative forcing of CH4

    International Nuclear Information System (INIS)

    Grossman, A.S.; Grant, K.E.

    1994-04-01

    We have evaluated the tropospheric radiative forcing of CH 4 in the 0-3000 cm -1 wavenumber range and compared this with prior published calculations. The atmospheric test cases involved perturbed methane scenarios in both a McClatchey mid latitude, summer, clear sky approximation, model atmosphere, as well as a globally and seasonally averaged model atmosphere containing a representative cloud distribution. The scenarios involved pure CH 4 radiative forcing and CH 4 plus a mixture of H 2 O, CO 2 , O 3 , and N 2 O. The IR radiative forcing was calculated using a correlated k-distribution transmission model. The major purposes of this paper are to first, use the correlated k-distribution model to calculate the tropospheric radiative forcing for CH 4 , as the only radiatively active gas, and in a mixture with H 2 O, CO 2 , O 3 , and N 2 O, for a McClatchey mid-latitude summer, clear-sky model atmosphere, and to compare the results to those obtained in the studies mentioned above. Second, we will calculate the tropospheric methane forcing in a globally and annually averaged atmosphere with and without a representative cloud distribution in order to validate the conjecture given in IPCC (1990) that the inclusion of clouds in the forcing calculations results in forcing values which are approximately 20 percent less than those obtained using clear sky approximations

  14. Tropospheric Enhancement of Ozone over the UAE

    Science.gov (United States)

    Abbasi, Naveed Ali; Majeed, Tariq; Iqbal, Mazhar; Kaminski, Jacek; Struzewska, Joanna; Durka, Pawel; Tarasick, David; Davies, Jonathan

    2015-04-01

    We use the Global Environmental Multiscale - Air Quality (GEM-AQ) model to interpret the vertical profiles of ozone acquired with ozone sounding experiments at the meteorological site located at the Abu Dhabi airport. The purpose of this study is to gain insight into the chemical and dynamical structures in the atmosphere of this unique subtropical location (latitude 24.45N; longitude 54.22E). Ozone observations for years 2012 - 2013 reveal elevated ozone abundances in the range from 70 ppbv to 120 ppbv near 500-400 hPa during summer. The ozone abundances in other seasons are much lower than these values. The preliminary results indicate that summertime enhancement in ozone is associated with the Arabian anticyclones centered over the Zagros Mountains in Iran and the Asir and Hijaz Mountain ranges in Saudi Arabia, and is consistent with TES observations of deuterated water. The model also shows considerable seasonal variation in the tropospheric ozone which is transported from the stratosphere by dynamical processes. The domestic production of ozone in the middle troposphere is estimated and compared GEM-AQ model. It is estimated that about 40-50% of ozone in the UAE is transported from the neighbouring petrochemical industries in the Gulf region. We will present ozone sounding data and GEM-AQ results including a discussion on the high levels of the tropospheric ozone responsible for contaminating the air quality in the UAE. This work is supported by National Research Foundation, UAE.

  15. Zonal management of arsenic contaminated ground water in Northwestern Bangladesh.

    Science.gov (United States)

    Hill, Jason; Hossain, Faisal; Bagtzoglou, Amvrossios C

    2009-09-01

    This paper used ordinary kriging to spatially map arsenic contamination in shallow aquifers of Northwestern Bangladesh (total area approximately 35,000 km(2)). The Northwestern region was selected because it represents a relatively safer source of large-scale and affordable water supply for the rest of Bangladesh currently faced with extensive arsenic contamination in drinking water (such as the Southern regions). Hence, the work appropriately explored sustainability issues by building upon a previously published study (Hossain et al., 2007; Water Resources Management, vol. 21: 1245-1261) where a more general nation-wide assessment afforded by kriging was identified. The arsenic database for reference comprised the nation-wide survey (of 3534 drinking wells) completed in 1999 by the British Geological Survey (BGS) in collaboration with the Department of Public Health Engineering (DPHE) of Bangladesh. Randomly sampled networks of zones from this reference database were used to develop an empirical variogram and develop maps of zonal arsenic concentration for the Northwestern region. The remaining non-sampled zones from the reference database were used to assess the accuracy of the kriged maps. Two additional criteria were explored: (1) the ability of geostatistical interpolators such as kriging to extrapolate information on spatial structure of arsenic contamination beyond small-scale exploratory domains; (2) the impact of a priori knowledge of anisotropic variability on the effectiveness of geostatistically based management. On the average, the kriging method was found to have a 90% probability of successful prediction of safe zones according to the WHO safe limit of 10ppb while for the Bangladesh safe limit of 50ppb, the safe zone prediction probability was 97%. Compared to the previous study by Hossain et al. (2007) over the rest of the contaminated country side, the probability of successful detection of safe zones in the Northwest is observed to be about 25

  16. Another look at zonal flows: Resonance, shearing, and frictionless saturation

    Science.gov (United States)

    Li, J. C.; Diamond, P. H.

    2018-04-01

    We show that shear is not the exclusive parameter that represents all aspects of flow structure effects on turbulence. Rather, wave-flow resonance enters turbulence regulation, both linearly and nonlinearly. Resonance suppresses the linear instability by wave absorption. Flow shear can weaken the resonance, and thus destabilize drift waves, in contrast to the near-universal conventional shear suppression paradigm. Furthermore, consideration of wave-flow resonance resolves the long-standing problem of how zonal flows (ZFs) saturate in the limit of weak or zero frictional drag, and also determines the ZF scale. We show that resonant vorticity mixing, which conserves potential enstrophy, enables ZF saturation in the absence of drag, and so is effective at regulating the Dimits up-shift regime. Vorticity mixing is incorporated as a nonlinear, self-regulation effect in an extended 0D predator-prey model of drift-ZF turbulence. This analysis determines the saturated ZF shear and shows that the mesoscopic ZF width scales as LZ F˜f3 /16(1-f ) 1 /8ρs5/8l03 /8 in the (relevant) adiabatic limit (i.e., τckk‖2D‖≫1 ). f is the fraction of turbulence energy coupled to ZF and l0 is the base state mixing length, absent ZF shears. We calculate and compare the stationary flow and turbulence level in frictionless, weakly frictional, and strongly frictional regimes. In the frictionless limit, the results differ significantly from conventionally quoted scalings derived for frictional regimes. To leading order, the flow is independent of turbulence intensity. The turbulence level scales as E ˜(γL/εc) 2 , which indicates the extent of the "near-marginal" regime to be γLcase of avalanche-induced profile variability. Here, εc is the rate of dissipation of potential enstrophy and γL is the characteristic linear growth rate of fluctuations. The implications for dynamics near marginality of the strong scaling of saturated E with γL are discussed.

  17. Tropospheric Emissions: Monitoring of Pollution (TEMPO)

    Science.gov (United States)

    Zoogman, P.; Liu, X.; Suleiman, R. M.; Pennington, W. F.; Flittner, D. E.; Al-Saadi, J. A.; Hilton, B. B.; Nicks, D. K.; Newchurch, M. J.; Carr, J. L.; hide

    2016-01-01

    TEMPO (Tropospheric Emissions: Monitoring of Pollution) was selected in 2012 by NASA as the first Earth Venture Instrument, for launch between 2018 and 2021. It will measure atmospheric pollution for greater North America from space using ultraviolet and visible spectroscopy. TEMPO observes from Mexico City, Cuba, and the Bahamas to the Canadian oil sands, and from the Atlantic to the Pacific, hourly and at high spatial resolution (approximately 2.1 kilometers N/S by 4.4 kilometers E/W at 36.5 degrees N, 100 degrees W). TEMPO provides a tropospheric measurement suite that includes the key elements of tropospheric air pollution chemistry, as well as contributing to carbon cycle knowledge. Measurements are made hourly from geostationary (GEO) orbit, to capture the high variability present in the diurnal cycle of emissions and chemistry that are unobservable from current low-Earth orbit (LEO) satellites that measure once per day. The small product spatial footprint resolves pollution sources at sub-urban scale. Together, this temporal and spatial resolution improves emission inventories, monitors population exposure, and enables effective emission-control strategies. TEMPO takes advantage of a commercial GEO host spacecraft to provide a modest cost mission that measures the spectra required to retrieve ozone (O3), nitrogen dioxide (NO2), sulfur dioxide (SO2), formaldehyde (H2CO), glyoxal (C2H2O2), bromine monoxide (BrO), IO (iodine monoxide),water vapor, aerosols, cloud parameters, ultraviolet radiation, and foliage properties. TEMPO thus measures the major elements, directly or by proxy, in the tropospheric O3 chemistry cycle. Multi-spectral observations provide sensitivity to O3 in the lowermost troposphere, substantially reducing uncertainty in air quality predictions. TEMPO quantifies and tracks the evolution of aerosol loading. It provides these near-real-time air quality products that will be made publicly available. TEMPO will launch at a prime time to be the

  18. Tropospheric Emissions: Monitoring of Pollution (TEMPO)

    Science.gov (United States)

    Chance, Kelly; Liu, Xiong; Suleiman, Raid M.; Flittner, David E.; Al-Saadi, Jassim; Janz, Scott J.

    2014-06-01

    TEMPO, selected by NASA as the first Earth Venture Instrument, will measure atmospheric pollution for greater North America from space using ultraviolet and visible spectroscopy. TEMPO measures from Mexico City to the Canadian oil sands, and from the Atlantic to the Pacific, hourly and at high spatial resolution. TEMPO provides a tropospheric measurement suite that includes the key elements of tropospheric air pollution chemistry. Measurements are from geostationary (GEO) orbit, to capture the inherent high variability in the diurnal cycle of emissions and chemistry. The small product spatial footprint resolves pollution sources at sub-urban scale. Together, this temporal and spatial resolution improves emission inventories, monitors population exposure, and enables effective emission-control strategies. TEMPO takes advantage of a GEO host spacecraft to provide a modest-cost mission that measures the spectra required to retrieve O3, NO2, SO2, H2CO, C2H2O2, H2O, aerosols, cloud parameters, and UVB radiation. TEMPO thus measures the major elements, directly or by proxy, in the tropospheric O3 chemistry cycle. Multi-spectral observations provide sensitivity to O3 in the lowermost troposphere, reducing uncertainty in air quality predictions by 50 %. TEMPO quantifies and tracks the evolution of aerosol loading. It provides near-real-time air quality products that will be made widely, publicly available. TEMPO makes the first tropospheric trace gas measurements from GEO, by building on the heritage of five spectrometers flown in low-earth-orbit (LEO). These LEO instruments measure the needed spectra, although at coarse spatial and temporal resolutions, to the precisions required for TEMPO and use retrieval algorithms developed for them by TEMPO Science Team members and currently running in operational environments. This makes TEMPO an innovative use of a well-proven technique, able to produce a revolutionary data set. TEMPO provides much of the atmospheric measurement

  19. Estimating zonal electricity supply curves in transmission-constrained electricity markets

    International Nuclear Information System (INIS)

    Sahraei-Ardakani, Mostafa; Blumsack, Seth; Kleit, Andrew

    2015-01-01

    Many important electricity policy initiatives would directly affect the operation of electric power networks. This paper develops a method for estimating short-run zonal supply curves in transmission-constrained electricity markets that can be implemented quickly by policy analysts with training in statistical methods and with publicly available data. Our model enables analysis of distributional impacts of policies affecting operation of electric power grid. The method uses fuel prices and zonal electric loads to determine piecewise supply curves, identifying zonal electricity price and marginal fuel. We illustrate our methodology by estimating zonal impacts of Pennsylvania's Act 129, an energy efficiency and conservation policy. For most utilities in Pennsylvania, Act 129 would reduce the influence of natural gas on electricity price formation and increase the influence of coal. The total resulted savings would be around 267 million dollars, 82 percent of which would be enjoyed by the customers in Pennsylvania. We also analyze the impacts of imposing a $35/ton tax on carbon dioxide emissions. Our results show that the policy would increase the average prices in PJM by 47–89 percent under different fuel price scenarios in the short run, and would lead to short-run interfuel substitution between natural gas and coal. - Highlights: • We develop a method to estimate of zonal supply curves in electricity markets. • The model estimates zonal electricity prices and zonal fuel utilization. • The model implicitly captures the average impacts of transmission constraints. • Using the method, we project supply curves for the seventeen utility zones of PJM. • We use the estimated supply curves to study the impacts of Pennsylvania's Act 129 and a carbon tax of $35 per ton

  20. Disturbance zonal and vertical plasma drifts in the Peruvian sector during solar minimum phases

    Science.gov (United States)

    Santos, A. M.; Abdu, M. A.; Souza, J. R.; Sobral, J. H. A.; Batista, I. S.

    2016-03-01

    In the present work, we investigate the behavior of the equatorial F region zonal plasma drifts over the Peruvian region under magnetically disturbed conditions during two solar minimum epochs, one of them being the recent prolonged solar activity minimum. The study utilizes the vertical and zonal components of the plasma drifts measured by the Jicamarca (11.95°S; 76.87°W) incoherent scatter radar during two events that occurred on 10 April 1997 and 24 June 2008 and model calculation of the zonal drift in a realistic ionosphere simulated by the Sheffield University Plasmasphere-Ionosphere Model-INPE. Two main points are focused: (1) the connection between electric fields and plasma drifts under prompt penetration electric field during a disturbed periods and (2) anomalous behavior of daytime zonal drift in the absence of any magnetic storm. A perfect anticorrelation between vertical and zonal drifts was observed during the night and in the initial and growth phases of the magnetic storm. For the first time, based on a realistic low-latitude ionosphere, we will show, on a detailed quantitative basis, that this anticorrelation is driven mainly by a vertical Hall electric field induced by the primary zonal electric field in the presence of an enhanced nighttime E region ionization. It is shown that an increase in the field line-integrated Hall-to-Pedersen conductivity ratio (∑H/∑P), which can arise from precipitation of energetic particles in the region of the South American Magnetic Anomaly, is capable of explaining the observed anticorrelation between the vertical and zonal plasma drifts. Evidence for the particle ionization is provided from the occurrence of anomalous sporadic E layers over the low-latitude station, Cachoeira Paulista (22.67°S; 44.9°W)—Brazil. It will also be shown that the zonal plasma drift reversal to eastward in the afternoon two hours earlier than its reference quiet time pattern is possibly caused by weakening of the zonal wind

  1. The role of zonal flows in the saturation of multi-scale gyrokinetic turbulence

    Energy Technology Data Exchange (ETDEWEB)

    Staebler, G. M.; Candy, J. [General Atomics, San Diego, California 92186 (United States); Howard, N. T. [Oak Ridge Institute for Science Education (ORISE), Oak Ridge, Tennessee 37831 (United States); Holland, C. [University of California San Diego, San Diego, California 92093 (United States)

    2016-06-15

    The 2D spectrum of the saturated electric potential from gyrokinetic turbulence simulations that include both ion and electron scales (multi-scale) in axisymmetric tokamak geometry is analyzed. The paradigm that the turbulence is saturated when the zonal (axisymmetic) ExB flow shearing rate competes with linear growth is shown to not apply to the electron scale turbulence. Instead, it is the mixing rate by the zonal ExB velocity spectrum with the turbulent distribution function that competes with linear growth. A model of this mechanism is shown to be able to capture the suppression of electron-scale turbulence by ion-scale turbulence and the threshold for the increase in electron scale turbulence when the ion-scale turbulence is reduced. The model computes the strength of the zonal flow velocity and the saturated potential spectrum from the linear growth rate spectrum. The model for the saturated electric potential spectrum is applied to a quasilinear transport model and shown to accurately reproduce the electron and ion energy fluxes of the non-linear gyrokinetic multi-scale simulations. The zonal flow mixing saturation model is also shown to reproduce the non-linear upshift in the critical temperature gradient caused by zonal flows in ion-scale gyrokinetic simulations.

  2. GRAVOTURBULENT PLANETESIMAL FORMATION: THE POSITIVE EFFECT OF LONG-LIVED ZONAL FLOWS

    International Nuclear Information System (INIS)

    Dittrich, K.; Klahr, H.; Johansen, A.

    2013-01-01

    Recent numerical simulations have shown long-lived axisymmetric sub- and super-Keplerian flows in protoplanetary disks. These zonal flows are found in local as well as global simulations of disks unstable to the magnetorotational instability. This paper covers our study of the strength and lifetime of zonal flows and the resulting long-lived gas over- and underdensities as functions of the azimuthal and radial size of the local shearing box. We further investigate dust particle concentrations without feedback on the gas and without self-gravity. The strength and lifetime of zonal flows increase with the radial extent of the simulation box, but decrease with the azimuthal box size. Our simulations support earlier results that zonal flows have a natural radial length scale of 5-7 gas pressure scale heights. This is the first study that combines three-dimensional MHD simulations of zonal flows and dust particles feeling the gas pressure. The pressure bumps trap particles with St = 1 very efficiently. We show that St = 0.1 particles (of some centimeters in size if at 5 AU in a minimum mass solar nebula) reach a hundred-fold higher density than initially. This opens the path for particles of St = 0.1 and dust-to-gas ratio of 0.01 or for particles of St ≥ 0.5 and dust-to-gas ratio 10 –4 to still reach densities that potentially trigger the streaming instability and thus gravoturbulent formation of planetesimals.

  3. Day-ahead optimal dispatch for wind integrated power system considering zonal reserve requirements

    International Nuclear Information System (INIS)

    Liu, Fan; Bie, Zhaohong; Liu, Shiyu; Ding, Tao

    2017-01-01

    Highlights: • Analyzing zonal reserve requirements for wind integrated power system. • Modeling day-ahead optimal dispatch solved by chance constrained programming theory. • Determining optimal zonal reserve demand with minimum confidence interval. • Analyzing numerical results on test and large-scale real-life power systems. - Abstract: Large-scale integration of renewable power presents a great challenge for day-ahead dispatch to manage renewable resources while provide available reserve for system security. Considering zonal reserve is an effective way to ensure reserve deliverability when network congested, a random day-ahead dispatch optimization of wind integrated power system for a least operational cost is modeled including zonal reserve requirements and N − 1 security constraints. The random model is transformed into a deterministic one based on the theory of chance constrained programming and a determination method of optimal zonal reserve demand is proposed using the minimum confidence interval. After solving the deterministic model, the stochastic simulation is conducted to verify the validity of solution. Numerical tests and results on the IEEE 39 bus system and a large-scale real-life power system demonstrate the optimal day-ahead dispatch scheme is available and the proposed method is effective for improving reserve deliverability and reducing load shedding after large-capacity power outage.

  4. Collisionless kinetic-fluid model of zonal flows in toroidal plasmas

    International Nuclear Information System (INIS)

    Sugama, H.; Watanabe, T.-H.; Horton, W.

    2006-12-01

    A novel kinetic-fluid model is presented, which describes collisionless time evolution of zonal flows in tokamaks. In the new zonal-flow closure relations, the parallel heat fluxes are written by the sum of short- and long-time-evolution parts. The former part is given in the dissipative form of the parallel heat diffusion and relates to collisionless damping processes. The latter is derived from the long-time-averaged gyrocenter distribution and plays a major role in describing low-frequency or stationary zonal flows, for which the parallel heat fluxes are expressed in terms of the parallel flow as well as the nonlinear-source and initial-condition terms. It is shown analytically and numerically that, when applied to the zonal flow driven by either ion or electron temperature gradient turbulence, the kinetic-fluid equations including the new closure relations can reproduce the same long-time zonal-flow responses to the initial condition and to the turbulence source as those obtained from the gyrokinetic model. (author)

  5. Tropospheric Ozone Climatology over Irene, South Africa, From 1990-1994 and 1998-2002

    Science.gov (United States)

    Diab, R. D.; Thompson, A. M.; Marl, K.; Ramsay, L.; Coetzee, G. J. R.

    2004-01-01

    This paper describes ozone profiles from sonde data during the period of NASA s TRACE-A and the more recent SHADOZ (Southern Hemisphere Additional Ozonesondes) period. The data were taken by the South African Weather Service at the Irene (25 deg.54 min S; 28 deg. 13 min. E) station near Pretoria, South Africa, an area that is a unique mixture of local industry, heavy biofuels use and importation of biomass burning ozone from neighboring countries to the north. The main findings are: (1) With its geographical position at the edge of the subtropical transition zone, mid- latitude dynamical influences are evident at Irene, predominantly in winter when upper tropospheric ozone is enhanced as a result of stratospheric-tropospheric exchange. (2) There has been an increase in the near-surface ozone amount between the early 1990s and a decade later, presumably due to an influx of rural population toward the Johannesburg-Pretoria area, as well as with industrial growth and development. (3) Most significant for developing approaches for satellite ozone profile climatologies, cluster analysis has enabled the delineation of a background and "most polluted" profile. Enhancements of at least 30% occur throughout the troposphere in spring and in certain layers increases of 100 % are observed.

  6. Sources of tropospheric ozone along the Asian Pacific Rim: An analysis of ozonesonde observations

    Science.gov (United States)

    Liu, Hongyu; Jacob, Daniel J.; Chan, Lo Yin; Oltmans, Samuel J.; Bey, Isabelle; Yantosca, Robert M.; Harris, Joyce M.; Duncan, Bryan N.; Martin, Randall V.

    2002-11-01

    The sources contributing to tropospheric ozone over the Asian Pacific Rim in different seasons are quantified by analysis of Hong Kong and Japanese ozonesonde observations with a global three-dimensional (3-D) chemical transport model (GEOS-CHEM) driven by assimilated meteorological observations. Particular focus is placed on the extensive observations available from Hong Kong in 1996. In the middle-upper troposphere (MT-UT), maximum Asian pollution influence along the Pacific Rim occurs in summer, reflecting rapid convective transport of surface pollution. In the lower troposphere (LT) the season of maximum Asian pollution influence shifts to summer at midlatitudes from fall at low latitudes due to monsoonal influence. The UT ozone minimum and high variability observed over Hong Kong in winter reflects frequent tropical intrusions alternating with stratospheric intrusions. Asian biomass burning makes a major contribution to ozone at pollution influence (pollution influence exceeds European influence in the UT-MT, reflecting the uplift from convection and the warm conveyor belts over the eastern seaboard of North America. African outflow makes a major contribution to ozone in the low-latitude MT-UT over the Pacific Rim during November-April. Lightning influence over the Pacific Rim is minimum in summer due to westward UT transport at low latitudes associated with the Tibetan anticyclone. The Asian outflow flux of ozone to the Pacific is maximum in spring and fall and includes a major contribution from Asian anthropogenic sources year-round.

  7. Tropospheric emissions: Monitoring of pollution (TEMPO)

    Science.gov (United States)

    Zoogman, P.; Liu, X.; Suleiman, R. M.; Pennington, W. F.; Flittner, D. E.; Al-Saadi, J. A.; Hilton, B. B.; Nicks, D. K.; Newchurch, M. J.; Carr, J. L.; Janz, S. J.; Andraschko, M. R.; Arola, A.; Baker, B. D.; Canova, B. P.; Chan Miller, C.; Cohen, R. C.; Davis, J. E.; Dussault, M. E.; Edwards, D. P.; Fishman, J.; Ghulam, A.; González Abad, G.; Grutter, M.; Herman, J. R.; Houck, J.; Jacob, D. J.; Joiner, J.; Kerridge, B. J.; Kim, J.; Krotkov, N. A.; Lamsal, L.; Li, C.; Lindfors, A.; Martin, R. V.; McElroy, C. T.; McLinden, C.; Natraj, V.; Neil, D. O.; Nowlan, C. R.; O`Sullivan, E. J.; Palmer, P. I.; Pierce, R. B.; Pippin, M. R.; Saiz-Lopez, A.; Spurr, R. J. D.; Szykman, J. J.; Torres, O.; Veefkind, J. P.; Veihelmann, B.; Wang, H.; Wang, J.; Chance, K.

    2017-01-01

    TEMPO was selected in 2012 by NASA as the first Earth Venture Instrument, for launch between 2018 and 2021. It will measure atmospheric pollution for greater North America from space using ultraviolet and visible spectroscopy. TEMPO observes from Mexico City, Cuba, and the Bahamas to the Canadian oil sands, and from the Atlantic to the Pacific, hourly and at high spatial resolution ( 2.1 km N/S×4.4 km E/W at 36.5°N, 100°W). TEMPO provides a tropospheric measurement suite that includes the key elements of tropospheric air pollution chemistry, as well as contributing to carbon cycle knowledge. Measurements are made hourly from geostationary (GEO) orbit, to capture the high variability present in the diurnal cycle of emissions and chemistry that are unobservable from current low-Earth orbit (LEO) satellites that measure once per day. The small product spatial footprint resolves pollution sources at sub-urban scale. Together, this temporal and spatial resolution improves emission inventories, monitors population exposure, and enables effective emission-control strategies. TEMPO takes advantage of a commercial GEO host spacecraft to provide a modest cost mission that measures the spectra required to retrieve ozone (O3), nitrogen dioxide (NO2), sulfur dioxide (SO2), formaldehyde (H2CO), glyoxal (C2H2O2), bromine monoxide (BrO), IO (iodine monoxide), water vapor, aerosols, cloud parameters, ultraviolet radiation, and foliage properties. TEMPO thus measures the major elements, directly or by proxy, in the tropospheric O3 chemistry cycle. Multi-spectral observations provide sensitivity to O3 in the lowermost troposphere, substantially reducing uncertainty in air quality predictions. TEMPO quantifies and tracks the evolution of aerosol loading. It provides these near-real-time air quality products that will be made publicly available. TEMPO will launch at a prime time to be the North American component of the global geostationary constellation of pollution monitoring

  8. Tropospheric Emissions: Monitoring of Pollution Overview

    Science.gov (United States)

    Chance, Kelly; Liu, Xiong; Suleiman, Raid M.; Flittner, David; Al-Saadi, Jay; Janz, Scott

    2015-01-01

    TEMPO is now well into its implementation phase, having passed both its Key Decision Point C and the Critical Design Review (CDR) for the instrument. The CDR for the ground systems will occur in March 2016 and the CDR for the Mission component at a later date, after the host spacecraft has been selected. TEMPO is on schedule to measure atmospheric pollution for greater North America from space using ultraviolet and visible spectroscopy. TEMPO measures from Mexico City to the Canadian oil sands, and from the Atlantic to the Pacific, hourly and at high spatial resolution. TEMPO provides a tropospheric measurement suite that includes the key elements of tropospheric air pollution chemistry. Measurements are from geostationary (GEO) orbit, to capture the inherent high variability in the diurnal cycle of emissions and chemistry. The small product spatial footprint resolves pollution sources at sub-urban scale. Together, this temporal and spatial resolution improves emission inventories, monitors population exposure, and enables effective emission-control strategies. TEMPO takes advantage of a GEO host spacecraft to provide a modest cost mission that measures the spectra required to retrieve O3, NO2, SO2, H2CO, C2H2O2, H2O, aerosols, cloud parameters, and UVB radiation. TEMPO thus measures the major elements, directly or by proxy, in the tropospheric O3 chemistry cycle. Multi-spectral observations provide sensitivity to O3 in the lowermost troposphere, substantially reducing uncertainty in air quality predictions by 50 percent. TEMPO quantifies and tracks the evolution of aerosol loading. It provides near-real-time air quality products that will be made widely, publicly available. TEMPO provides much of the atmospheric measurement capability recommended for GEO-CAPE in the 2007 National Research Council Decadal Survey, Earth Science and Applications from Space: National Imperatives for the Next Decade and Beyond. Instruments from Europe (Sentinel 4) and Asia (GEMS) will

  9. Longitudinal variability in Jupiter's zonal winds derived from multi-wavelength HST observations

    Science.gov (United States)

    Johnson, Perianne E.; Morales-Juberías, Raúl; Simon, Amy; Gaulme, Patrick; Wong, Michael H.; Cosentino, Richard G.

    2018-06-01

    Multi-wavelength Hubble Space Telescope (HST) images of Jupiter from the Outer Planets Atmospheres Legacy (OPAL) and Wide Field Coverage for Juno (WFCJ) programs in 2015, 2016, and 2017 are used to derive wind profiles as a function of latitude and longitude. Wind profiles are typically zonally averaged to reduce measurement uncertainties. However, doing this destroys any variations of the zonal-component of winds in the longitudinal direction. Here, we present the results derived from using a "sliding-window" correlation method. This method adds longitudinal specificity, and allows for the detection of spatial variations in the zonal winds. Spatial variations are identified in two jets: 1 at 17 ° N, the location of a prominent westward jet, and the other at 7 ° S, the location of the chevrons. Temporal and spatial variations at the 24°N jet and the 5-μm hot spots are also examined.

  10. Nonlinear saturation of the slab ITG instability and zonal flow generation with fully kinetic ions

    Science.gov (United States)

    Miecnikowski, Matthew T.; Sturdevant, Benjamin J.; Chen, Yang; Parker, Scott E.

    2018-05-01

    Fully kinetic turbulence models are of interest for their potential to validate or replace gyrokinetic models in plasma regimes where the gyrokinetic expansion parameters are marginal. Here, we demonstrate fully kinetic ion capability by simulating the growth and nonlinear saturation of the ion-temperature-gradient instability in shearless slab geometry assuming adiabatic electrons and including zonal flow dynamics. The ion trajectories are integrated using the Lorentz force, and the cyclotron motion is fully resolved. Linear growth and nonlinear saturation characteristics show excellent agreement with analogous gyrokinetic simulations across a wide range of parameters. The fully kinetic simulation accurately reproduces the nonlinearly generated zonal flow. This work demonstrates nonlinear capability, resolution of weak gradient drive, and zonal flow physics, which are critical aspects of modeling plasma turbulence with full ion dynamics.

  11. Zonally averaged model of dynamics, chemistry and radiation for the atmosphere

    Science.gov (United States)

    Tung, K. K.

    1985-01-01

    A nongeostrophic theory of zonally averaged circulation is formulated using the nonlinear primitive equations on a sphere, taking advantage of the more direct relationship between the mean meridional circulation and diabatic heating rate which is available in isentropic coordinates. Possible differences between results of nongeostrophic theory and the commonly used geostrophic formulation are discussed concerning: (1) the role of eddy forcing of the diabatic circulation, and (2) the nonlinear nearly inviscid limit vs the geostrophic limit. Problems associated with the traditional Rossby number scaling in quasi-geostrophic formulations are pointed out and an alternate, more general scaling based on the smallness of mean meridional to zonal velocities for a rotating planet is suggested. Such a scaling recovers the geostrophic balanced wind relationship for the mean zonal flow but reveals that the mean meridional velocity is in general ageostrophic.

  12. Effects of plasma current on nonlinear interactions of ITG turbulence, zonal flows and geodesic acoustic modes

    International Nuclear Information System (INIS)

    Angelino, P; Bottino, A; Hatzky, R; Jolliet, S; Sauter, O; Tran, T M; Villard, L

    2006-01-01

    The mutual interactions of ion temperature gradient (ITG) driven modes, zonal flows and geodesic acoustic modes (GAM) in tokamak plasmas are investigated using a global nonlinear gyrokinetic formulation with totally unconstrained evolution of temperature gradient and profile. A series of numerical simulations with the same initial temperature and density profile specifications is performed using a sequence of ideal MHD equilibria differing only in the value of the total plasma current, in particular with identical magnetic shear profiles and shapes of magnetic surfaces. On top of a bursty or quasi-steady state behaviour the zonal flows oscillate at the GAM frequency. The amplitude of these oscillations increases with the value of the safety factor q, resulting in a less effective suppression of ITG turbulence by zonal flows at a lower plasma current. The turbulence-driven volume-averaged radial heat transport is found to scale inversely with the total plasma current

  13. The influence of regional Arctic sea-ice decline on stratospheric and tropospheric circulation

    Science.gov (United States)

    McKenna, Christine; Bracegirdle, Thomas; Shuckburgh, Emily; Haynes, Peter

    2016-04-01

    region (one perturbation experiment combines all regions). These regions correspond to sea-ice loss hotspots such as the Barents-Kara Seas and the Bering Sea. The differences between the control and perturbation runs yields the effects of the imposed sea-ice loss on the polar vortex. To detect and count SSWs for each run, we use the World Meteorological Organisation's definition of an SSW (a reversal in zonal mean zonal wind at 10 hPa and 60° N, and a reversal in zonal mean meridional temperature gradient at 10 hPa between 60° N and 90° N). The poster will present and discuss the initial results of this study. Implications of the results for future change in the lower latitude mid-troposphere will be discussed. References Sun, L., C. Deser, and R. A. Tomas, 2015: Mechanisms of Stratospheric and Tropospheric Circulation Response to Projected Arctic Sea Ice Loss. J. Climate, 28, 7824-7845, doi: http://dx.doi.org/10.1175/JCLI-D-15-0169.1.

  14. Zonal NePhRO scoring system: a superior renal tumor complexity classification model.

    Science.gov (United States)

    Hakky, Tariq S; Baumgarten, Adam S; Allen, Bryan; Lin, Hui-Yi; Ercole, Cesar E; Sexton, Wade J; Spiess, Philippe E

    2014-02-01

    Since the advent of the first standardized renal tumor complexity system, many subsequent scoring systems have been introduced, many of which are complicated and can make it difficult to accurately measure data end points. In light of these limitations, we introduce the new zonal NePhRO scoring system. The zonal NePhRO score is based on 4 anatomical components that are assigned a score of 1, 2, or 3, and their sum is used to classify renal tumors. The zonal NePhRO scoring system is made up of the (Ne)arness to collecting system, (Ph)ysical location of the tumor in the kidney, (R)adius of the tumor, and (O)rganization of the tumor. In this retrospective study, we evaluated patients exhibiting clinical stage T1a or T1b who underwent open partial nephrectomy performed by 2 genitourinary surgeons. Each renal unit was assigned both a zonal NePhRO score and a RENAL (radius, exophytic/endophytic properties, nearness of tumor to the collecting system or sinus in millimeters, anterior/posterior, location relative to polar lines) score, and a blinded reviewer used the same preoperative imaging study to obtain both scores. Additional data points gathered included age, clamp time, complication rate, urine leak rate, intraoperative blood loss, and pathologic tumor size. One hundred sixty-six patients underwent open partial nephrectomy. There were 37 perioperative complications quantitated using the validated Clavien-Dindo system; their occurrence was predicted by the NePhRO score on both univariate and multivariate analyses (P = .0008). Clinical stage, intraoperative blood loss, and tumor diameter were all correlated with the zonal NePhRO score on univariate analysis only. The zonal NePhRO scoring system is a simpler tool that accurately predicts the surgical complexity of a renal lesion. Copyright © 2014 Elsevier Inc. All rights reserved.

  15. Low-frequency variation of a zonally localized jet stream: Observation and theory

    International Nuclear Information System (INIS)

    Cai, M.

    1994-01-01

    The climatological mean circulation in the extratropics of the Northern Hemisphere is characterized by two zonally localized jet streams over the east coasts of the two major continents. The zonal inhomogeneity of the climatological mean circulation is believed to be a primary factor determining the geographical locations of the maximum activity centers of the atmospheric transients, such as storm tracks over the east coasts of the two major continents and frequent blocking episodes occurring over the central regions of the two oceans. The impact of the transients on the zonally localized jet streams is studied mostly in the linear dynamics framework in terms of so-called open-quotes feedbackclose quotes diagnosis. This study investigates nonlinear instability of a zonally localized jet stream. The emphasis is on the nonlinear adjustment of a zonally localized jet stream associated with the development of the transients via local instability. The adjustment of a zonally localized jet stream would naturally consists of two parts: One is the time-invariant part and the other is the transient part (temporal variation of the adjustment). In conjunction with the observation, the time-mean adjustment is part of the climatological mean flow and hence is open-quotes invisible.close quotes The transient part of the adjustment is evidenced by the changes of the jet streams in terms of both location and intensity. In this study, we tend to relate the transient part of the adjustment of the jet stream to the maximum activity centers of low-frequency variability. The underlying mechanisms that are responsible for the temporal variation of the adjustment will be investigated. The time-mean adjustment will be also studied to better understand the temporal variation of the adjustment

  16. Kinetics programs for simulation of tropospheric photochemistry on the global scale

    International Nuclear Information System (INIS)

    Elliott, S.; Kao, C.Y.J.; Turco, R.P.; Zhao, X.P.

    1993-08-01

    The study of tropospheric kinetics underlies global change because key greenhouse gases are photochemically active. Modeling of tropospheric chemistry on a global scale is essential because some indirect greenhouse gases are short-lived and interact in a non-linear fashion. It is also extremely challenging, however; the global change grid is extensive in both the physical and temporal domains, and critical lower atmospheric species include the organics and their oxidized derivatives, which are numerous. Several types of optimization may be incorporated into kinetics modules to enhance their ability to simulate the complete lower atmospheric gas phase chemical system. (1) The photochemical integrator can be accelerated by avoiding matrix and iterative solutions and by establishing families. Accuracy and mass conservation are sacrificed in the absence of iteration, but atom balancing is restorable post hoc. (2) Chemistry can be arranged upon the massive grid to exploit parallel processing, and solutions to its continuity equations can be automated to permit experimentation with species and reaction lists or family definitions. Costs in programming effort will be incurred in these cases. (3) Complex hydrocarbon decay sequences can be streamlined either through structural lumping methods descended from smog investigations, which require considerable calibration, or by defining surrogates for classes of compounds, with a loss in constituent detail. From among the available options, the most advantageous permutations will vary with the specific nature of any eventual global scale study, and there is likely to be demand for many approaches. Tracer transport codes serve as a foundation upon which tropospheric chemistry packages will be tested. Encroachment of the NO x sphere of influence upon tropical rain forests and the upper free troposphere are two examples of specific problems to which full three-dimensional chemical simulations might be applied

  17. Evaluating the lower-tropospheric COSMIC GPS radio occultation sounding quality over the Arctic

    Science.gov (United States)

    Yu, Xiao; Xie, Feiqin; Ao, Chi O.

    2018-04-01

    Lower-tropospheric moisture and temperature measurements are crucial for understanding weather prediction and climate change. Global Positioning System radio occultation (GPS RO) has been demonstrated as a high-quality observation technique with high vertical resolution and sub-kelvin temperature precision from the upper troposphere to the stratosphere. In the tropical lower troposphere, particularly the lowest 2 km, the quality of RO retrievals is known to be degraded and is a topic of active research. However, it is not clear whether similar problems exist at high latitudes, particularly over the Arctic, which is characterized by smooth ocean surface and often negligible moisture in the atmosphere. In this study, 3-year (2008-2010) GPS RO soundings from COSMIC (Constellation Observing System for Meteorology, Ionosphere, and Climate) over the Arctic (65-90° N) show uniform spatial sampling with average penetration depth within 300 m above the ocean surface. Over 70 % of RO soundings penetrate deep into the lowest 300 m of the troposphere in all non-summer seasons. However, the fraction of such deeply penetrating profiles reduces to only about 50-60 % in summer, when near-surface moisture and its variation increase. Both structural and parametric uncertainties of GPS RO soundings were also analyzed. The structural uncertainty (due to different data processing approaches) is estimated to be within ˜ 0.07 % in refractivity, ˜ 0.72 K in temperature, and ˜ 0.05 g kg-1 in specific humidity below 10 km, which is derived by comparing RO retrievals from two independent data processing centers. The parametric uncertainty (internal uncertainty of RO sounding) is quantified by comparing GPS RO with near-coincident radiosonde and European Centre for Medium-Range Weather Forecasts (ECMWF) ERA-Interim profiles. A systematic negative bias up to ˜ 1 % in refractivity below 2 km is only seen in the summer, which confirms the moisture impact on GPS RO quality.

  18. Effects of anthropogenic emissions on tropospheric ozone and its radiative forcing

    Energy Technology Data Exchange (ETDEWEB)

    Berntsen, T.; Isaksen, I.S.A.; Fuglestvedt, J.S.; Myhre, G.; Larsen, T. Alsvik; Stordal, F.; Freckleton, R.S.; Shine, K.P.

    1997-12-31

    As described in this report, changes in tropospheric ozone since pre-industrial times due to changes in emissions have been calculated by the University of Oslo global three-dimensional photochemical model. The radiative forcing caused by the increase in ozone has been calculated by means of two independent radiative transfer models: the University of Reading model (Reading), and the University of Oslo/Norwegian Institute for Air Research model (OsloRad). Significant increases in upper tropospheric ozone concentrations are found at northern mid-latitudes at about 10 km altitude. In the tropical regions the largest increase is found at about 15 km altitude. The increase is found to be caused mainly by enhanced in situ production due to transport of precursors from the boundary layer, with a smaller contribution from increased transport of ozone produced in the boundary layer. The lifetime of ozone in the troposphere decreased by about 35% as a result of enhanced concentrations of HO{sub 2}. The calculated increase in surface ozone in Europe is in good agreement with observations. The calculations of radiative forcing include the effect of clouds and allow for thermal adjustment in the stratosphere. The global and annual averaged radiative forcing at the tropopause from both models are in the lower part of the Intergovernmental Panel on Climate Change estimated range. The calculated radiative forcing is similar in magnitude to the negative radiative forcing by sulfate aerosols, but displaced southward in source regions at northern mid-latitudes. The increase in tropospheric ozone is calculated to have cooled the lower stratosphere by up to 0.9 K, with possibly half of this cooling occurring in the past 2 to 3 decades. 76 refs., 16 figs., 9 tabs.

  19. Comparison of Global Distributions of Zonal-Mean Gravity Wave Variance Inferred from Different Satellite Instruments

    Science.gov (United States)

    Preusse, Peter; Eckermann, Stephen D.; Offermann, Dirk; Jackman, Charles H. (Technical Monitor)

    2000-01-01

    Gravity wave temperature fluctuations acquired by the CRISTA instrument are compared to previous estimates of zonal-mean gravity wave temperature variance inferred from the LIMS, MLS and GPS/MET satellite instruments during northern winter. Careful attention is paid to the range of vertical wavelengths resolved by each instrument. Good agreement between CRISTA data and previously published results from LIMS, MLS and GPS/MET are found. Key latitudinal features in these variances are consistent with previous findings from ground-based measurements and some simple models. We conclude that all four satellite instruments provide reliable global data on zonal-mean gravity wave temperature fluctuations throughout the middle atmosphere.

  20. Gyrokinetic simulations in general geometry and applications to collisional damping of zonal flows

    International Nuclear Information System (INIS)

    Lin, Z.; Hahm, T.S.; Lee, W.W.; Tang, W.M.; White, R.B.

    2000-01-01

    A fully three-dimensional gyrokinetic particle code using magnetic coordinates for general geometry has been developed and applied to the investigation of zonal flows dynamics in toroidal ion-temperature-gradient turbulence. Full torus simulation results support the important conclusion that turbulence-driven zonal flows significantly reduce the turbulent transport. Linear collisionless simulations for damping of an initial poloidal flow perturbation exhibit an asymptotic residual flow. The collisional damping of this residual causes the dependence of ion thermal transport on the ion-ion collision frequency even in regimes where the instabilities are collisionless

  1. Effects of regional-scale and convective transports on tropospheric ozone chemistry revealed by aircraft observations during the wet season of the AMMA campaign

    Directory of Open Access Journals (Sweden)

    G. Ancellet

    2009-01-01

    Full Text Available The African Monsoon Multidisciplinary Analyses (AMMA fourth airborne campaign was conducted in July–August 2006 to study the chemical composition of the middle and upper troposphere in West Africa with the major objective to better understand the processing of chemical emissions by the West African Monsoon (WAM and its associated regional-scale and vertical transports. In particular, the french airborne experiment was organized around two goals. The first was to characterize the impact of Mesoscale Convective Systems (MCSs on the ozone budget in the upper troposphere and the evolution of the chemical composition of these convective plumes as they move westward toward the Atlantic Ocean. The second objective was to discriminate the impact of remote sources of pollution over West Africa, including transport from the middle east, Europe, Asia and from southern hemispheric fires. Observations of O3, CO, NOx, H2O and hydroperoxide above West Africa along repeated meridional transects were coupled with transport analysis based on the FLEXPART lagrangian model. The cross analysis of trace gas concentrations and transport pathways revealed 5 types of air masses: convective uplift of industrial and urban emissions, convective uplift of biogenic emissions, slow advection from Cotonou polluted plumes near the coast, meridional transport of upper tropospheric air from the subtropical barrier region, and meridional transport of Southern Hemisphere (SH biomass burning emissions. O3/CO correlation plots and the correlation plots of H2O2 with a OH proxy revealed not only a control of the trace gas variability by transport processes but also significant photochemical reactivity in the mid- and upper troposphere. The study of four MCSs outflow showed contrasted chemical composition and air mass origins depending on the MCSs lifetime and latitudinal position. Favorables conditions for ozone

  2. Rapid increases in tropospheric ozone production and export from China

    NARCIS (Netherlands)

    Verstraeten, W.W.; Neu, J.L.; Williams, J.E.; Bowman, K.W.; Worden, J.R.; Boersma, K.F.

    2015-01-01

    Rapid population growth and industrialization have driven substantial increases in Asian ozone precursor emissions over the past decade1, with highly uncertain impacts on regional and global tropospheric ozone levels. According to ozonesonde measurements2, 3, tropospheric ozone concentrations at two

  3. Role of upper-level wind shear on the structure and maintenance of derecho-producing convective systems

    Science.gov (United States)

    Coniglio, Michael Charles

    Common large-scale environments associated with the development of derecho-producing convective systems from a large number of events are identified using statistical clustering of the 500-mb geopotential heights as guidance. The majority of the events (72%) fall into three main patterns that include a well-defined upstream trough (40%), a ridge (20%), and a zonal, low-amplitude flow (12%), which is defined as an additional warm-season pattern that is not identified in past studies of derecho environments. Through an analysis of proximity soundings, discrepancies are found in both low-level and deep-tropospheric shear parameters between observations and the shear profiles considered favorable for strong, long-lived convective systems in idealized simulations. To explore the role of upper-level shear in derecho environments, a set of two-dimensional simulations of density currents within a dry, neutrally stable environment are used to examine the ability of a cold pool to lift environmental air within a vertically sheared flow. The results confirm that the addition of upper-level shear to a wind profile with weak to moderate low-level shear increases the vertical displacement of low-level parcels despite a decrease in the vertical velocity along the cold pool interface, as suggested by previous studies. Parcels that are elevated above the surface (1-2 km) overturn and are responsible for the deep lifting in the deep-shear environments. This deep overturning caused by the upper-level shear helps to maintain the tilt of the convective systems in more complex two-dimensional and three dimensional simulations. The overturning also is shown to greatly increase the size of the convective systems in the three-dimensional simulations by facilitating the initiation and maintenance of convective cells along the cold pool. When combined with estimates of the cold pool motion and the storm-relative hodograph, these results may best be used for the prediction of the demise of

  4. The influence of biogenic emissions from Africa on tropical tropospheric ozone during 2006: a global modeling study

    Directory of Open Access Journals (Sweden)

    J. E. Williams

    2009-08-01

    Full Text Available We have performed simulations using a 3-D global chemistry-transport model to investigate the influence that biogenic emissions from the African continent exert on the composition of the troposphere in the tropical region. For this purpose we have applied two recently developed biogenic emission inventories provided for use in large-scale global models (Granier et al., 2005; Lathière et al., 2006 whose seasonality and temporal distribution for biogenic emissions of isoprene, other volatile organic compounds and NO is markedly different. The use of the 12 year average values for biogenic emissions provided by Lathière et al. (2006 results in an increase in the amount of nitrogen sequestrated into longer lived reservoir compounds which contributes to the reduction in the tropospheric ozone burden in the tropics. The associated re-partitioning of nitrogen between PAN, HNO3 and organic nitrates also results in a ~5% increase in the loss of nitrogen by wet deposition. At a global scale there is a reduction in the oxidizing capacity of the model atmosphere which increases the atmospheric lifetimes of CH4 and CO by ~1.5% and ~4%, respectively. Comparisons against a range of different measurements indicate that applying the 12 year average of Lathière et al. (2006 improves the performance of TM4_AMMA for 2006 in the tropics. By the use of sensitivity studies we show that the release of NO from soils in Africa accounts for between ~2–45% of tropospheric ozone in the African troposphere, ~10% in the upper troposphere and between ~5–20% of the tropical tropospheric ozone column over the tropical Atlantic Ocean. The subsequent reduction in OH over the source regions allows enhanced transport of CO out of the region. For biogenic volatile organic C1 to C3 species released from Africa, the effects on tropical tropospheric ozone are rather limited, although this source contributes to the global burden of VOC by between ~2–4% and

  5. [Altitude-belt zonality of wood vegetation within mountainous regions of the Sayan Mountains: a model of ecological second-order phase transitions ].

    Science.gov (United States)

    Sukhovol'skiĭ, V G; Ovchinnikova, T M; Baboĭ, S D

    2014-01-01

    As a description of altitude-belt zonality of wood vegetation, a model of ecological second-order transitions is proposed. Objects of the study have been chosen to be forest cenoses of the northern slope of Kulumyss Ridge (the Sayan Mauntains), while the results are comprised by the altitude profiles of wood vegetation. An ecological phase transition can be considered as the transition of cenoses at different altitudes from the state of presence of certain tree species within the studied territory to the state of their absence. By analogy with the physical model of second-order, phase transitions the order parameter is introduced (i.e., the area portion occupied by a single tree species at the certain altitude) as well as the control variable (i.e., the altitude of the wood vegetation belt). As the formal relation between them, an analog of the Landau's equation for phase transitions in physical systems is obtained. It is shown that the model is in a good accordance with the empirical data. Thus, the model can be used for estimation of upper and lower boundaries of altitude belts for individual tree species (like birch, aspen, Siberian fir, Siberian pine) as well as the breadth of their ecological niches with regard to altitude. The model includes also the parameters that describe numerically the interactions between different species of wood vegetation. The approach versatility allows to simplify description and modeling of wood vegetation altitude zonality, and enables assessment of vegetation cenoses response to climatic changes.

  6. Efficient transport of tropospheric aerosol into the stratosphere via the Asian summer monsoon anticyclone

    Science.gov (United States)

    Yu, Pengfei; Rosenlof, Karen H.; Liu, Shang; Telg, Hagen; Thornberry, Troy D.; Rollins, Andrew W.; Portmann, Robert W.; Bai, Zhixuan; Ray, Eric A.; Duan, Yunjun; Pan, Laura L.; Toon, Owen B.; Bian, Jianchun; Gao, Ru-Shan

    2017-07-01

    An enhanced aerosol layer near the tropopause over Asia during the June-September period of the Asian summer monsoon (ASM) was recently identified using satellite observations. Its sources and climate impact are presently not well-characterized. To improve understanding of this phenomenon, we made in situ aerosol measurements during summer 2015 from Kunming, China, then followed with a modeling study to assess the global significance. The in situ measurements revealed a robust enhancement in aerosol concentration that extended up to 2 km above the tropopause. A climate model simulation demonstrates that the abundant anthropogenic aerosol precursor emissions from Asia coupled with rapid vertical transport associated with monsoon convection leads to significant particle formation in the upper troposphere within the ASM anticyclone. These particles subsequently spread throughout the entire Northern Hemispheric (NH) lower stratosphere and contribute significantly (˜15%) to the NH stratospheric column aerosol surface area on an annual basis. This contribution is comparable to that from the sum of small volcanic eruptions in the period between 2000 and 2015. Although the ASM contribution is smaller than that from tropical upwelling (˜35%), we find that this region is about three times as efficient per unit area and time in populating the NH stratosphere with aerosol. With a substantial amount of organic and sulfur emissions in Asia, the ASM anticyclone serves as an efficient smokestack venting aerosols to the upper troposphere and lower stratosphere. As economic growth continues in Asia, the relative importance of Asian emissions to stratospheric aerosol is likely to increase.

  7. Light microscopical demonstration and zonal distribution of parasinusoidal cells (Ito cells) in normal human liver

    DEFF Research Database (Denmark)

    Horn, T; Junge, Jette; Nielsen, O

    1988-01-01

    The parasinusoidal cells of the liver (Ito cells) were demonstrated light microscopically in autopsy specimens fixed in formalin and stained with Oil red O after dichromate treatment. The method allows examination of large samples containing numerous acini. Quantitative assessment showed a zonal...

  8. Numerical simulation of phenomenon on zonal disintegration in deep underground mining in case of unsupported roadway

    Science.gov (United States)

    Han, Fengshan; Wu, Xinli; Li, Xia; Zhu, Dekang

    2018-02-01

    Zonal disintegration phenomenon was found in deep mining roadway surrounding rock. It seriously affects the safety of mining and underground engineering and it may lead to the occurrence of natural disasters. in deep mining roadway surrounding rock, tectonic stress in deep mining roadway rock mass, horizontal stress is much greater than the vertical stress, When the direction of maximum principal stress is parallel to the axis of the roadway in deep mining, this is the main reasons for Zonal disintegration phenomenon. Using ABAQUS software to numerical simulation of the three-dimensional model of roadway rupture formation process systematically, and the study shows that when The Direction of maximum main stress in deep underground mining is along the roadway axial direction, Zonal disintegration phenomenon in deep underground mining is successfully reproduced by our numerical simulation..numerical simulation shows that using ABAQUA simulation can reproduce Zonal disintegration phenomenon and the formation process of damage of surrounding rock can be reproduced. which have important engineering practical significance.

  9. Multi-scale-nonlinear interactions among micro-turbulence, double tearing instability and zonal flows

    International Nuclear Information System (INIS)

    Ishizawa, A.; Nakajima, N.

    2007-01-01

    Micro-turbulence and macro-magnetohydrodynamic (macro-MHD) instabilities can appear in plasma at the same time and interact with each other in a plasma confinement. The multi-scale-nonlinear interaction among micro-turbulence, double tearing instability and zonal flow is investigated by numerically solving a reduced set of two-fluid equations. It is found that the double tearing instability, which is a macro-MHD instability, appears in an equilibrium formed by a balance between micro-turbulence and zonal flow when the double tearing mode is unstable. The roles of the nonlinear and linear terms of the equations in driving the zonal flow and coherent convective cell flow of the double tearing mode are examined. The Reynolds stress drives zonal flow and coherent convective cell flow, while the ion diamagnetic term and Maxwell stress oppose the Reynolds stress drive. When the double tearing mode grows, linear terms in the equations are dominant and they effectively release the free energy of the equilibrium current gradient

  10. Pole dynamics for the Flierl-Petvishvili equation and zonal flow

    International Nuclear Information System (INIS)

    Spineanu, F.; Vlad, M.; Itoh, K.; Sanuki, H.; Itoh, S.-I.

    2003-09-01

    We use a systematic method which allows us to identify a class of exact solutions of the Flierl-Petvishvili equation. The solutions are periodic and have one dimensional geometry. We examine the physical properties and find that these structures can have a significant effect on the zonal flow generation. (author)

  11. Elaboration of generalized criterion for zonality determination of the Chernobyl' NPP working spaces

    International Nuclear Information System (INIS)

    Simakov, A.V.; Bad'in, V.I.; Nosovskij, A.V.

    1992-01-01

    Analysis of the features of radioactive dose rating, regularities of their formation and dosimetry allows suggesting generalized criterion for assess zonality of compartments and territories, combining all factors and their action on operators. This criterion may be used during design of the new objects, development of programs and pursuance of work on removal of atomic power plants from operation. 6 refs.; 1 fig

  12. Light microscopical demonstration and zonal distribution of parasinusoidal cells (Ito cells) in normal human liver

    DEFF Research Database (Denmark)

    Horn, T; Junge, Jette; Nielsen, O

    1988-01-01

    The parasinusoidal cells of the liver (Ito cells) were demonstrated light microscopically in autopsy specimens fixed in formalin and stained with Oil red O after dichromate treatment. The method allows examination of large samples containing numerous acini. Quantitative assessment showed a zonal ...

  13. Nonlinear generation of zonal flows by ion-acoustic waves in a uniform magnetoplasma

    International Nuclear Information System (INIS)

    Shukla, Nitin; Shukla, P.K.

    2010-01-01

    It is shown that large-scale zonal flows (ZFs) can be excited by Reynolds stress of nonlinearly interacting random phase ion-acoustic waves (EIAWs) in a uniform magnetoplasma. Since ZFs are associated with poloidal sheared flows, they can tear apart short scale EIAW turbulence eddies, and hence contribute to the reduction of the cross-field turbulent transport in a magnetized plasma.

  14. The paramo vegetation of Ramal de Guaramacal, Trujillo State, Venezuela. 1. Zonal communities

    NARCIS (Netherlands)

    Cuello, A.N.L.; Cleef, A.M.

    2009-01-01

    Zonal paramo vegetation communities present on top of Ramal de Guaramacal, Trujillo state, Venezuela, have been studied with the aim to provide a syntaxonomic scheme or classification, based oil analysis of the physiognomy, floristic composition, ecological relations and spatial distribution of the

  15. Simulations of Tokamak Edge Turbulence Including Self-Consistent Zonal Flows

    Science.gov (United States)

    Cohen, Bruce; Umansky, Maxim

    2013-10-01

    Progress on simulations of electromagnetic drift-resistive ballooning turbulence in the tokamak edge is summarized in this mini-conference talk. A more detailed report on this work is presented in a poster at this conference. This work extends our previous work to include self-consistent zonal flows and their effects. The previous work addressed the simulation of L-mode tokamak edge turbulence using the turbulence code BOUT. The calculations used realistic single-null geometry and plasma parameters of the DIII-D tokamak and produced fluctuation amplitudes, fluctuation spectra, and particle and thermal fluxes that compare favorably to experimental data. In the effect of sheared ExB poloidal rotation is included with an imposed static radial electric field fitted to experimental data. In the new work here we include the radial electric field self-consistently driven by the microturbulence, which contributes to the sheared ExB poloidal rotation (zonal flow generation). We present simulations with/without zonal flows for both cylindrical geometry, as in the UCLA Large Plasma Device, and for the DIII-D tokamak L-mode cases in to quantify the influence of self-consistent zonal flows on the microturbulence and the concomitant transport. This work was performed under the auspices of the US Department of Energy under contract DE-AC52-07NA27344 at the Lawrence Livermore National Laboratory.

  16. Simulations of Turbulence in Tokamak Edge and Effects of Self-Consistent Zonal Flows

    Science.gov (United States)

    Cohen, Bruce; Umansky, Maxim

    2013-10-01

    Progress is reported on simulations of electromagnetic drift-resistive ballooning turbulence in the tokamak edge. This extends previous work to include self-consistent zonal flows and their effects. The previous work addressed simulation of L-mode tokamak edge turbulence using the turbulence code BOUT that solves Braginskii-based plasma fluid equations in tokamak edge domain. The calculations use realistic single-null geometry and plasma parameters of the DIII-D tokamak and produce fluctuation amplitudes, fluctuation spectra, and particle and thermal fluxes that compare favorably to experimental data. In the effect of sheared ExB poloidal rotation is included with an imposed static radial electric field fitted to experimental data. In the new work here we include the radial electric field self-consistently driven by the microturbulence, which contributes to the sheared ExB poloidal rotation (zonal flow generation). We present simulations with/without zonal flows for both cylindrical geometry, as in the UCLA Large Plasma Device, and for the DIII-D tokamak L-mode cases in to quantify the influence of self-consistent zonal flows on the microturbulence and the concomitant transport. This work was performed under the auspices of the U.S. Department of Energy under contract DE-AC52-07NA27344 at the Lawrence Livermore National Laboratory.

  17. Analysis of zonal flow bifurcations in 3D drift wave turbulence simulations

    International Nuclear Information System (INIS)

    Kammel, Andreas

    2012-01-01

    The main issue of experimental magnetic fusion devices lies with their inherently high turbulent transport, preventing long-term plasma confinement. A deeper understanding of the underlying transport processes is therefore desirable, especially in the high-gradient tokamak edge which marks the location of the drift wave regime as well as the outer boundary of the still badly understood high confinement mode. One of the most promising plasma features possibly connected to a complete bifurcation theory for the transition to this H-mode is found in large-scale phenomena capable of regulating radial transport through vortex shearing - i.e. zonal flows, linearly stable large-scale poloidal vector E x vector B-modes based on radial flux surface averages of the potential gradient generated through turbulent self-organization. Despite their relevance, few detailed turbulence studies of drift wave-based zonal flows have been undertaken, and none of them have explicitly targeted bifurcations - or, within a resistive sheared-slab environment, observed zonal flows at all. In this work, both analytical means and the two-fluid code NLET are used to analyze a reduced set of Hasegawa-Wakatani equations, describing a sheared collisional drift wave system without curvature. The characteristics of the drift waves themselves, as well as those of the drift wave-based zonal flows and their retroaction on the drift wave turbulence are examined. The single dimensionless parameter ρ s proposed in previous analytical models is examined numerically and shown to divide the drift wave scale into two transport regimes, the behavioral characteristics of which agree perfectly with theoretical expectations. This transport transition correlates with a transition from pure drift wave turbulence at low ρ s into the high-ρ s zonal flow regime. The associated threshold has been more clearly identified by tracing it back to a tipping of the ratio between a newly proposed frequency gradient length at

  18. Theoretical and experimental zonal drift velocities of the ionospheric plasma bubbles over the Brazilian region

    Science.gov (United States)

    Arruda, Daniela C. S.; Sobral, J. H. A.; Abdu, M. A.; Castilho, Vivian M.; Takahashi, H.; Medeiros, A. F.; Buriti, R. A.

    2006-01-01

    This work presents equatorial ionospheric plasma bubble zonal drift velocity observations and their comparison with model calculations. The bubble zonal velocities were measured using airglow OI630 nm all-sky digital images and the model calculations were performed taking into account flux-tube integrated Pedersen conductivity and conductivity weighted neutral zonal winds. The digital images were obtained from an all-sky imaging system operated over the low-latitude station Cachoeira Paulista (Geogr. 22.5S, 45W, dip angle 31.5S) during the period from October 1998 to August 2000. Out of the 138 nights of imager observation, 29 nights with the presence of plasma bubbles are used in this study. These 29 nights correspond to geomagnetically rather quiet days (∑K P hours, the calculated zonal drift velocities were found to be larger than the experimental values. The best matching between the calculated and observed zonal velocities were seen to be for a few hours around midnight. The model calculation showed two humps around 20 LT and 24 LT that were not present in the data. Average decelerations obtained from linear regression between 20 LT and 24 LT were found to be: (a) Spring 1998, -8.61 ms -1 h -1; (b) Summer 1999, -0.59 ms -1 h -1; (c) Spring 1999, -11.72 ms -1 h -1; and (d) Summer 2000, -8.59 ms -1 h -1. Notice that Summer and Winter here correspond to southern hemisphere Summer and Winter, not northern hemisphere.

  19. Measuring tropospheric wind with microwave sounders

    Science.gov (United States)

    Lambrigtsen, B.; Su, H.; Turk, J.; Hristova-Veleva, S. M.; Dang, V. T.

    2017-12-01

    In its 2007 "Decadal Survey" of earth science missions for NASA the U.S. National Research Council recommended that a Doppler wind lidar be developed for a three-dimensional tropospheric winds mission ("3D-Winds"). The technology required for such a mission has not yet been developed, and it is expected that the next Decadal Survey, planned to be released by the end of 2017, will put additional emphasis on the still pressing need for wind measurements from space. The first Decadal Survey also called for a geostationary microwave sounder (GMS) on a Precipitation and All-weather Temperature and Humidity (PATH) mission, which could be used to measure wind from space. Such a sounder, the Geostationary Synthetic Thinned Aperture Radiometer (GeoSTAR), has been developed at the Jet Propulsion Laboratory (JPL). The PATH mission has not yet been funded by NASA, but a low-cost subset of PATH, GeoStorm has been proposed as a hosted payload on a commercial communications satellite. Both PATH and GeoStorm would obtain frequent (every 15 minutes of better) measurements of tropospheric water vapor profiles, and they can be used to derive atmospheric motion vector (AMV) wind profiles, even in the presence of clouds. Measurement of wind is particularly important in the tropics, where the atmosphere is largely not in thermal balance and wind estimates cannot generally be derived from temperature and pressure fields. We report on simulation studies of AMV wind vectors derived from a GMS and from a cluster of low-earth-orbiting (LEO) small satellites (e.g., CubeSats). The results of two separate simulation studies are very encouraging and show that a ±2 m/s wind speed precision is attainable, which would satisfy WMO requirements. A GMS observing system in particular, which can be implemented now, would enable significant progress in the study of atmospheric dynamics. Copyright 2017 California Institute of Technology. Government sponsorship acknowledged

  20. Impact of the new HNO3-forming channel of the HO2+NO reaction on tropospheric HNO3, NOx, HOx and ozone

    Directory of Open Access Journals (Sweden)

    A. Kukui

    2008-07-01

    Full Text Available We have studied the impact of the recently observed reaction NO+HO2→HNO3 on atmospheric chemistry. A pressure and temperature-dependent parameterisation of this minor channel of the NO+HO2→NO2+OH reaction has been included in both a 2-D stratosphere-troposphere model and a 3-D tropospheric chemical transport model (CTM. Significant effects on the nitrogen species and hydroxyl radical concentrations are found throughout the troposphere, with the largest percentage changes occurring in the tropical upper troposphere (UT. Including the reaction leads to a reduction in NOx everywhere in the troposphere, with the largest decrease of 25% in the tropical and Southern Hemisphere UT. The tropical UT also has a corresponding large increase in HNO3 of 25%. OH decreases throughout the troposphere with the largest reduction of over 20% in the tropical UT. The mean global decrease in OH is around 13%, which is very large compared to the impact that typical photochemical revisions have on this modelled quantity. This OH decrease leads to an increase in CH4 lifetime of 5%. Due to the impact of decreased NOx on the OH:HO2 partitioning, modelled HO2 actually increases in the tropical UT on including the new reaction. The impact on tropospheric ozone is a decrease in the range 5 to 12%, with the largest impact in the tropics and Southern Hemisphere. Comparison with observations shows that in the region of largest changes, i.e. the tropical UT, the inclusion of the new reaction tends to degrade the model agreement. Elsewhere the model comparisons are not able to critically assess the impact of including this reaction. Only small changes are calculated in the minor species distributions in the stratosphere.

  1. Is tropospheric weather influenced by solar wind through atmospheric vertical coupling downward control?

    Science.gov (United States)

    Prikryl, Paul; Tsukijihara, Takumi; Iwao, Koki; Muldrew, Donald B.; Bruntz, Robert; Rušin, Vojto; Rybanský, Milan; Turňa, Maroš; Šťastný, Pavel; Pastirčák, Vladimír

    2017-04-01

    More than four decades have passed since a link between solar wind magnetic sector boundary structure and mid-latitude upper tropospheric vorticity was discovered (Wilcox et al., Science, 180, 185-186, 1973). The link has been later confirmed and various physical mechanisms proposed but apart from controversy, little attention has been drawn to these results. To further emphasize their importance we investigate the occurrence of mid-latitude severe weather in the context of solar wind coupling to the magnetosphere-ionosphere-atmosphere (MIA) system. It is observed that significant snowstorms, windstorms and heavy rain, particularly if caused by low pressure systems in winter, tend to follow arrivals of high-speed solar wind. Previously published statistical evidence that explosive extratropical cyclones in the northern hemisphere tend to occur after arrivals of high-speed solar wind streams from coronal holes (Prikryl et al., Ann. Geophys., 27, 1-30, 2009; Prikryl et al., J. Atmos. Sol.-Terr. Phys., 149, 219-231, 2016) is corroborated for the southern hemisphere. A physical mechanism to explain these observations is proposed. The leading edge of high-speed solar wind streams is a locus of large-amplitude magneto-hydrodynamic waves that modulate Joule heating and/or Lorentz forcing of the high-latitude lower thermosphere generating medium-scale atmospheric gravity waves that propagate upward and downward through the atmosphere. Simulations of gravity wave propagation in a model atmosphere using the Transfer Function Model (Mayr et al., Space Sci. Rev., 54, 297-375, 1990) show that propagating waves originating in the thermosphere can excite a spectrum of gravity waves in the lower atmosphere. In spite of significantly reduced amplitudes but subject to amplification upon reflection in the upper troposphere, these gravity waves can provide a lift of unstable air to release instabilities in the troposphere thus initiating convection to form cloud/precipitation bands

  2. Photochemistry and transport of tropospheric ozone and its precursors in urban and remote environments

    Science.gov (United States)

    Anderson, Daniel Craig

    Tropospheric ozone (O3) adversely affects human health, reduces crop yields, and contributes to climate forcing. To limit these effects, the processes controlling O3 abundance as well as that of its precursor molecules must be fully characterized. Here, I examine three facets of O 3 production, both in heavily polluted and remote environments. First, using in situ observations from the DISCOVER-AQ field campaign in the Baltimore/Washington region, I evaluate the emissions of the O 3 precursors CO and NOx (NOx = NO + NO2) in the National Emissions Inventory (NEI). I find that CO/NOx emissions ratios derived from observations are 21% higher than those predicted by the NEI. Comparisons to output from the CMAQ model suggest that CO in the NEI is accurate within 15 +/- 11%, while NOx emissions are overestimated by 51-70%, likely due to errors in mobile sources. These results imply that ambient ozone concentrations will respond more efficiently to NOx controls than current models suggest. I then investigate the source of high O3 and low H2O structures in the Tropical Western Pacific (TWP). A combination of in situ observations, satellite data, and models show that the high O3 results from photochemical production in biomass burning plumes from fires in tropical Southeast Asia and Central Africa; the low relative humidity results from large-scale descent in the tropics. Because these structures have frequently been attributed to mid-latitude pollution, biomass burning in the tropics likely contributes more to the radiative forcing of climate than previously believed. Finally, I evaluate the processes controlling formaldehyde (HCHO) in the TWP. Convective transport of near surface HCHO leads to a 33% increase in upper tropospheric HCHO mixing ratios; convection also likely increases upper tropospheric CH 3OOH to ~230 pptv, enough to maintain background HCHO at ~75 pptv. The long-range transport of polluted air, with NO four times the convectively controlled background

  3. Tropospheric mercury vertical profiles between 500 and 10 000 m in central Europe

    Directory of Open Access Journals (Sweden)

    A. Weigelt

    2016-03-01

    Full Text Available The knowledge of the vertical distribution of atmospheric mercury (Hg plays an important role in determining the transport and cycling of mercury. However, measurements of the vertical distribution are rare, because airborne measurements are expensive and labour intensive. Consequently, only a few vertical Hg profile measurements have been reported since the 1970s. Besides the Civil Aircraft for the Regular Investigation of the atmosphere Based on an Instrument Container (CARIBIC observations, the latest vertical profile over Europe was measured in 1996. Within the Global Mercury Observation System (GMOS project, four vertical profiles were taken on board research aircraft (CASA-212 in August 2013 in background air over different locations in Slovenia and Germany. Each vertical profile consists of at least seven 5 min horizontal flight sections from 500 m above ground to 3000 m a.s.l. Gaseous elemental mercury (GEM and total gaseous mercury (TGM were measured with Tekran 2537X and Tekran 2537B analysers. In addition to the mercury measurements, SO2, CO, O3, NO, and NO2, basic meteorological parameters (pressure, temperature, relative humidity have been measured. Additional ground-based mercury measurements at the GMOS master site in Waldhof, Germany and measurements onboard the CARIBIC passenger aircraft were used to extend the profile to the ground and upper troposphere respectively. No vertical gradient was found inside the well-mixed boundary layer (variation of less than 0.1 ng m−3 at different sites, with GEM varying from location to location between 1.4 and 1.6 ng m−3 (standard temperature and pressure, STP: T  =  273.15 K, p  =  1013.25 hPa. At all locations GEM dropped to 1.3 ng m−3 (STP when entering the free troposphere and remained constant at higher altitudes. The combination of the vertical profile, measured on 21 August 2013 over Leipzig, Germany, with the CARIBIC measurements during ascent and descent to

  4. Chemical and aerosol characterisation of the troposphere over West Africa during the monsoon period as part of AMMA

    Directory of Open Access Journals (Sweden)

    C. E. Reeves

    2010-08-01

    Full Text Available During June, July and August 2006 five aircraft took part in a campaign over West Africa to observe the aerosol content and chemical composition of the troposphere and lower stratosphere as part of the African Monsoon Multidisciplinary Analysis (AMMA project. These are the first such measurements in this region during the monsoon period. In addition to providing an overview of the tropospheric composition, this paper provides a description of the measurement strategy (flights performed, instrumental payloads, wing-tip to wing-tip comparisons and points to some of the important findings discussed in more detail in other papers in this special issue.

    The ozone data exhibits an "S" shaped vertical profile which appears to result from significant losses in the lower troposphere due to rapid deposition to forested areas and photochemical destruction in the moist monsoon air, and convective uplift of ozone-poor air to the upper troposphere. This profile is disturbed, particularly in the south of the region, by the intrusions in the lower and middle troposphere of air from the southern hemisphere impacted by biomass burning. Comparisons with longer term data sets suggest the impact of these intrusions on West Africa in 2006 was greater than in other recent wet seasons. There is evidence for net photochemical production of ozone in these biomass burning plumes as well as in urban plumes, in particular that from Lagos, convective outflow in the upper troposphere and in boundary layer air affected by nitrogen oxide emissions from recently wetted soils. This latter effect, along with enhanced deposition to the forested areas, contributes to a latitudinal gradient of ozone in the lower troposphere. Biogenic volatile organic compounds are also important in defining the composition both for the boundary layer and upper tropospheric convective outflow.

    Mineral dust was found to be the most abundant and ubiquitous aerosol type in the

  5. Uncertainty in the Future Distribution of Tropospheric Ozone over West Africa due to Variability in Anthropogenic Emissions Estimates between 2025 and 2050

    Directory of Open Access Journals (Sweden)

    J. E. Williams

    2011-01-01

    Full Text Available Particle and trace gas emissions due to anthropogenic activity are expected to increase significantly in West Africa over the next few decades due to rising population and more energy intensive lifestyles. Here we perform 3D global chemistry-transport model calculations for 2025 and 2050 using both a “business-as-usual” (A1B and “clean economy” (B1 future anthropogenic emission scenario to focus on the changes in the distribution and uncertainties associated with tropospheric O3 due to the various projected emission scenarios. When compared to the present-day troposphere we find that there are significant increases in tropospheric O3 for the A1B emission scenario, with the largest increases being located in the lower troposphere near the source regions and into the Sahel around 15–20°N. In part this increase is due to more efficient NOx re-cycling related to increases in the background methane concentrations. Examining the uncertainty across different emission inventories reveals that there is an associated uncertainty of up to ~20% in the predicted increases at 2025 and 2050. For the upper troposphere, where increases in O3 have a more pronounced impact on radiative forcing, the uncertainty is influenced by transport of O3 rich air from Asia on the Tropical Easterly Jet.

  6. Anisotropic turbulence and zonal jets in rotating flows with a β-effect

    Directory of Open Access Journals (Sweden)

    B. Galperin

    2006-01-01

    Full Text Available Numerical studies of small-scale forced, two-dimensional turbulent flows on the surface of a rotating sphere have revealed strong large-scale anisotropization that culminates in the emergence of quasi-steady sets of alternating zonal jets, or zonation. The kinetic energy spectrum of such flows also becomes strongly anisotropic. For the zonal modes, a steep spectral distribution, E(n=CZ (Ω/R2 n-5, is established, where CZ=O(1 is a non-dimensional coefficient, Ω is the angular velocity, and R is the radius of the sphere, respectively. For other, non-zonal modes, the classical, Kolmogorov-Batchelor-Kraichnan, spectral law is preserved. This flow regime, referred to as a zonostrophic regime, appears to have wide applicability to large-scale planetary and terrestrial circulations as long as those are characterized by strong rotation, vertically stable stratification and small Burger numbers. The well-known manifestations of this regime are the banded disks of the outer planets of our Solar System. Relatively less known examples are systems of narrow, subsurface, alternating zonal jets throughout all major oceans discovered in state-of-the-art, eddy-permitting simulations of the general oceanic circulation. Furthermore, laboratory experiments recently conducted using the Coriolis turntable have basically confirmed that the lateral gradient of ''planetary vorticity'' (emulated via the topographic β-effect is the primary cause of the zonation and that the latter is entwined with the development of the strongly anisotropic kinetic energy spectrum that tends to attain the same zonal and non-zonal distributions, −5 and , respectively, in both the slope and the magnitude, as the corresponding spectra in other environmental conditions. The non-dimensional coefficient CZ in the −5 spectral law appears to be invariant, , in a variety of simulated and natural flows. This paper provides a brief review of the zonostrophic regime. The review includes the

  7. Vertical distribution and sources of tropospheric ozone over South China in spring 2004: Ozonesonde measurements and modeling analysis

    Science.gov (United States)

    Zhang, Y.; Liu, H.; Crawford, J. H.; Considine, D. B.; Chan, C.; Scientific Team Of Tapto

    2010-12-01

    The Transport of Air Pollutant and Tropospheric Ozone over China (TAPTO-China) science initiative is a two-year (TAPTO 2004 and 2005) field measurement campaign to help improve our understanding of the physical and chemical processes that control the tropospheric ozone budget over the Chinese subcontinent (including the Asian Pacific rim) and its surrounding SE Asia. In this paper, we use two state-of-the-art 3-D global chemical transport models (GEOS-Chem and Global Modeling Initiative or GMI) to examine the characteristics of vertical distribution and quantify the sources of tropospheric ozone by analysis of TAPTO in-situ ozonesonde data obtained at five stations in South China during spring (April and May) 2004: Lin’an (30.30N, 119.75E), Tengchong (25.01N, 98.30E), Taipei (25.0N, 121.3E), Hong Kong (22.21N, 114.30E) and Sanya (18.21N, 110.31E). The observed tropospheric ozone concentrations show strong spatial and temporal variability, which is largely captured by the models. The models simulate well the observed vertical gradients of tropospheric ozone at higher latitudes but are too low at lower latitudes. Model tagged ozone simulations suggest that stratosphere has a large impact on the upper and middle troposphere (UT/MT) at Lin’an and Tengchong. Continental SE Asian biomass burning emissions are maximum in March but still contribute significantly to the photochemical production of tropopheric ozone in South China in early April. Asian anthropogenic emissions are the major contribution to lower tropospheric ozone at all stations. On the other hand, there are episodes of influence from European/North American anthropogenic emissions. For example, model tagged ozone simulations show that over Lin’an in April 2004, stratosphere contributes 20% (13 ppbv) at 5 km, Asian boundary layer contributes 70% (46 ppbv) to ozone in the boundary layer, European boundary layer contributes 5% (3-4 ppbv) at 1.2 km, and North American boundary layer contributes 4.5% (3

  8. Blob/hole formation and zonal-flow generation in the edge plasma of the JET tokamak

    DEFF Research Database (Denmark)

    Xu, G.S.; Naulin, Volker; Fundamenski, W.

    2009-01-01

    The first experimental evidence showing the connection between blob/hole formation and zonal-flow generation was obtained in the edge plasma of the JET tokamak. Holes as well as blobs are observed to be born in the edge shear layer, where zonal-flows shear off meso-scale coherent structures......, leading to disconnection of positive and negative pressure perturbations. The newly formed blobs transport azimuthal momentum up the gradient of the azimuthal flow and drive the zonal-flow shear while moving outwards. During this process energy is transferred from the meso-scale coherent structures...

  9. Analysis of the tropospheric water distribution during FIRE 2

    Science.gov (United States)

    Westphal, Douglas L.

    1993-01-01

    The Penn State/NCAR mesoscale model, as adapted for use at ARC, was used as a testbed for the development and validation of cloud models for use in General Circulation Models (GCM's). This modeling approach also allows us to intercompare the predictions of the various cloud schemes within the same dynamical framework. The use of the PSU/NCAR mesoscale model also allows us to compare our results with FIRE-II (First International Satellite Cloud Climatology Project Regional Experiment) observations, instead of climate statistics. Though a promising approach, our work to date revealed several difficulties. First, the model by design is limited in spatial coverage and is only run for 12 to 48 hours at a time. Hence the quality of the simulation will depend heavily on the initial conditions. The poor quality of upper-tropospheric measurements of water vapor is well known and the situation is particularly bad for mid-latitude winter since the coupling with the surface is less direct than in summer so that relying on the model to spin-up a reasonable moisture field is not always successful. Though one of the most common atmospheric constituents, water vapor is relatively difficult to measure accurately, especially operationally over large areas. The standard NWS sondes have little sensitivity at the low temperatures where cirrus form and the data from the GOES 6.7 micron channel is difficult to quantify. For this reason, the goals of FIRE Cirrus II included characterizing the three-dimensional distribution of water vapor and clouds. In studying the data from FIRE Cirrus II, it was found that no single special observation technique provides accurate regional distributions of water vapor. The Raman lidar provides accurate measurements, but only at the Hub, for levels up to 10 km, and during nighttime hours. The CLASS sondes are more sensitive to moisture at low temperatures than are the NWS sondes, but the four stations only cover an area of two hundred kilometers on a side

  10. Variable influence on the equatorial troposphere associated with ...

    Indian Academy of Sciences (India)

    sphere to the stratosphere due to the uneven land profile (Matsuno ... an impact of the North Atlantic ocean-atmosphere heat flux, Eurasian ... convective clouds in the stratosphere–troposphere dynamics ..... modeling benchmarks; J. Clim.

  11. Verification and Validation of Tropospheric Model/Database

    National Research Council Canada - National Science Library

    Junho, choi

    1998-01-01

    A verification and validation of tropospheric models and databases has been performed based on ray tracing algorithm, statistical analysis, test on real time system operation, and other technical evaluation process...

  12. MSU (Microwave Sounding Unit) Daily Troposphere Temperatures and Precipitation

    Data.gov (United States)

    National Oceanic and Atmospheric Administration, Department of Commerce — This data set consists of two MSU tropospheric temperatures levels and precipitation which are described in detail below. The NOAA satellites contributing to this...

  13. Derivation of Tropospheric Ozone Climatology and Trends from TOMS Data

    Science.gov (United States)

    Newchurch, Michael J.; McPeters, Rich; Logan, Jennifer; Kim, Jae-Hwan

    2002-01-01

    This research addresses the following three objectives: (1) Derive tropospheric ozone columns from the TOMS instruments by computing the difference between total-ozone columns over cloudy areas and over clear areas in the tropics; (2) Compute secular trends in Nimbus-7 derived tropospheric Ozone column amounts and associated potential trends in the decadal-scale tropical cloud climatology; (3) Explain the occurrence of anomalously high ozone retrievals over high ice clouds.

  14. Impact of land convection on troposphere-stratosphere exchange in the tropics

    Directory of Open Access Journals (Sweden)

    P. Ricaud

    2007-11-01

    Full Text Available The mechanism of troposphere-stratosphere exchange in the tropics was investigated from space-borne observations of the horizontal distributions of tropospheric-origin long-lived species, nitrous oxide (N2O, methane (CH4 and carbon monoxide (CO, from 150 to 70 hPa in March-April-May by the ODIN/Sub-Millimeter Radiometer (SMR, the Upper Atmosphere Research Satellite (UARS/Halogen Occultation Experiment (HALOE and the TERRA/Measurements Of Pollution In The Troposphere (MOPITT instruments in 2002–2004, completed by recent observations of the AURA/Microwave Limb Sounder (MLS instrument during the same season in 2005. The vertical resolution of the satellite measurements ranges from 2 to 4 km. The analysis has been performed on isentropic surfaces: 400 K (lower stratosphere for all the species and 360 K (upper troposphere only for CO. At 400 K (and 360 K for CO, all gases show significant longitudinal variations with peak-to-trough values of ~5–11 ppbv for N2O, 0.07–0.13 ppmv for CH4, and ~10 ppbv for CO (~40 ppbv at 360 K. The maximum amounts are primarily located over Africa and, depending on the species, secondary more or less pronounced maxima are reported above northern South America and South-East Asia. The lower stratosphere over the Western Pacific deep convective region where the outgoing longwave radiation is the lowest, the tropopause the highest and the coldest, appears as a region of minimum concentration of tropospheric trace species. The possible impact on trace gas concentration at the tropopause of the inhomogeneous distribution and intensity of the sources, mostly continental, of the horizontal and vertical transports in the troposphere, and of cross-tropopause transport was explored with the MOCAGE Chemistry Transport Model. In the simulations, significant longitudinal variations were found on the medium-lived CO (2-month lifetime with peak-to-trough value of ~20 ppbv at 360 K and

  15. Measuring Zonal Transport Variability of the Antarctic Circumpolar Current Using GRACE Ocean Bottom Pressure

    Science.gov (United States)

    Makowski, J.; Chambers, D. P.; Bonin, J. A.

    2012-12-01

    Previous studies have suggested that ocean bottom pressure (OBP) can be used to measure the transport variability of the Antarctic Circumpolar Current (ACC). Using OBP data from the JPL ECCO model and the Gravity Recovery and Climate Experiment (GRACE), we examine the zonal transport variability of the ACC integrated between the major fronts between 2003-2010. The JPL ECCO data are used to determine average front positions for the time period studies, as well as where transport is mainly zonal. Statistical analysis will be conducted to determine the uncertainty of the GRACE observations using a simulated data set. We will also begin looking at low frequency changes and how coherent transport variability is from region to region of the ACC. Correlations with bottom pressure south of the ACC and the average basin transports will also be calculated to determine the probability of using bottom pressure south of the ACC as a means for describing the ACC dynamics and transport.

  16. Zonal wavefront sensing using a grating array printed on a polyester film

    Science.gov (United States)

    Pathak, Biswajit; Kumar, Suraj; Boruah, Bosanta R.

    2015-12-01

    In this paper, we describe the development of a zonal wavefront sensor that comprises an array of binary diffraction gratings realized on a transparent sheet (i.e., polyester film) followed by a focusing lens and a camera. The sensor works in a manner similar to that of a Shack-Hartmann wavefront sensor. The fabrication of the array of gratings is immune to certain issues associated with the fabrication of the lenslet array which is commonly used in zonal wavefront sensing. Besides the sensing method offers several important advantages such as flexible dynamic range, easy configurability, and option to enhance the sensing frame rate. Here, we have demonstrated the working of the proposed sensor using a proof-of-principle experimental arrangement.

  17. Zonal wavefront sensing using a grating array printed on a polyester film

    Energy Technology Data Exchange (ETDEWEB)

    Pathak, Biswajit; Boruah, Bosanta R., E-mail: brboruah@iitg.ernet.in [Department of Physics, Indian Institute of Technology Guwahati, Guwahati, Assam 781039 (India); Kumar, Suraj [Department of Applied Sciences, Gauhati University, Guwahati, Assam 781014 (India)

    2015-12-15

    In this paper, we describe the development of a zonal wavefront sensor that comprises an array of binary diffraction gratings realized on a transparent sheet (i.e., polyester film) followed by a focusing lens and a camera. The sensor works in a manner similar to that of a Shack-Hartmann wavefront sensor. The fabrication of the array of gratings is immune to certain issues associated with the fabrication of the lenslet array which is commonly used in zonal wavefront sensing. Besides the sensing method offers several important advantages such as flexible dynamic range, easy configurability, and option to enhance the sensing frame rate. Here, we have demonstrated the working of the proposed sensor using a proof-of-principle experimental arrangement.

  18. Using a Zonal Model To Assess the Effect of a Heated Floor on Thermal Comfort Quality

    International Nuclear Information System (INIS)

    Boukhris, Yosr; Gharbi, Leila; Ghrab-Morcos, Nadia

    2009-01-01

    People s perceptions of indoor air quality and thermal comfort are affected by air speed and temperature. We have extended the three-dimensional zonal model, ZAER, to be able to predict the temperature fields and the air distributions between and within rooms in the case of natural convection. This paper presents an application of the new zonal model dealing with the influence of a heated floor of one room upon the winter thermal comfort of an unconditioned Tunisian dwelling. Coupling ZAER with a thermal comfort model allows the assessment of the thermal quality of the dwelling through the prediction of a comfort indicator. The obtained results show that a heated floor can be a useful component to improve thermal comfort in the Tunisian context, even in another room

  19. Numerical study of unsteady flows past oscillating airfoils using direct zonal coupling method

    International Nuclear Information System (INIS)

    Zhang, F.; Khalid, M.

    2005-01-01

    A direct zonal coupling method was proposed for solving the flows past oscillating airfoils in this study. The entire computational domain was divided into inner and outer zones. The grid in the inner zone is moving with the oscillation of the airfoil, whereas the grid in the outer zone is artificially adjusted to the position consistent with the inner zone grid. The governing equations in the moving frame (the rotation potential energy is included) and those under the stationary frame were applied to inner and outer zones, respectively. By using this kind of treatment, the grid on the zonal interface is 1-to-1 matched. The coupling between the two zones is direct. Both the geometric and flow conservations are entirely satisfied. The NACA0012 and NLR7301 airfoils with oscillations were used as the test cases. The accuracy of the proposed method was demonstrated by the computational results compared with the experimental data.(author)

  20. (abstract) Tropospheric Calibration for the Mars Observer Gravity Wave Experiment

    Science.gov (United States)

    Walter, Steven J.; Armstrong, John

    1994-01-01

    In spring 1993, microwave radiometer-based tropospheric calibration was provided for the Mars Observer gravitational wave search. The Doppler shifted X-band radio signals propagating between Earth and the Mars Observer satellite were precisely measured to determine path length variations that might signal passage of gravitational waves. Experimental sensitivity was restricted by competing sources of variability in signal transit time. Principally, fluctuations in the solar wind and ionospheric plasma density combined with fluctions in tropospheric refractivity determined the detection limit. Troposphere-induced path delay fluctions are dominated by refractive changes caused by water vapor inhomogeneities blowing through the signal path. Since passive microwave remote sensing techniques are able to determine atmospheric propagation delays, radiometer-based tropospheric calibration was provided at the Deep Space Network Uranus tracking site (DSS-15). Two microwave water vapor radiometers (WVRs), a microwave temperature profiler (MTP), and a ground based meterological station were deployed to determine line-of-sight vapor content and vertical temperature profile concurrently with Mars Observer tracking measurements. This calibration system provided the capability to correct Mars Observer Doppler data for troposphere-induced path variations. We present preliminary analysis of the Doppler and WVR data sets illustrating the utility of WVRs to calibrate Doppler data. This takes an important step toward realizing the ambitious system required to support future Ka-band Cassini satellite gravity wave tropospheric calibration system.

  1. Climatology of tropospheric vertical velocity spectra

    Science.gov (United States)

    Ecklund, W. L.; Gage, K. S.; Balsley, B. B.; Carter, D. A.

    1986-01-01

    Vertical velocity power spectra obtained from Poker Flat, Alaska; Platteville, Colorado; Rhone Delta, France; and Ponape, East Caroline Islands using 50-MHz clear-air radars with vertical beams are given. The spectra were obtained by analyzing the quietest periods from the one-minute-resolution time series for each site. The lengths of available vertical records ranged from as long as 6 months at Poker Flat to about 1 month at Platteville. The quiet-time vertical velocity spectra are shown. Spectral period ranging from 2 minutes to 4 hours is shown on the abscissa and power spectral density is given on the ordinate. The Brunt-Vaisala (B-V) periods (determined from nearby sounding balloons) are indicated. All spectra (except the one from Platteville) exhibit a peak at periods slightly longer than the B-V period, are flat at longer periods, and fall rapidly at periods less than the B-V period. This behavior is expected for a spectrum of internal waves and is very similar to what is observed in the ocean (Eriksen, 1978). The spectral amplitudes vary by only a factor of 2 or 3 about the mean, and show that under quiet conditions vertical velocity spectra from the troposphere are very similar at widely different locations.

  2. A new diagnostic for tropospheric ozone production

    Science.gov (United States)

    Edwards, Peter M.; Evans, Mathew J.

    2017-11-01

    Tropospheric ozone is important for the Earth's climate and air quality. It is produced during the oxidation of organics in the presence of nitrogen oxides. Due to the range of organic species emitted and the chain-like nature of their oxidation, this chemistry is complex and understanding the role of different processes (emission, deposition, chemistry) is difficult. We demonstrate a new methodology for diagnosing ozone production based on the processing of bonds contained within emitted molecules, the fate of which is determined by the conservation of spin of the bonding electrons. Using this methodology to diagnose ozone production in the GEOS-Chem chemical transport model, we demonstrate its advantages over the standard diagnostic. We show that the number of bonds emitted, their chemistry and lifetime, and feedbacks on OH are all important in determining the ozone production within the model and its sensitivity to changes. This insight may allow future model-model comparisons to better identify the root causes of model differences.

  3. A new diagnostic for tropospheric ozone production

    Directory of Open Access Journals (Sweden)

    P. M. Edwards

    2017-11-01

    Full Text Available Tropospheric ozone is important for the Earth's climate and air quality. It is produced during the oxidation of organics in the presence of nitrogen oxides. Due to the range of organic species emitted and the chain-like nature of their oxidation, this chemistry is complex and understanding the role of different processes (emission, deposition, chemistry is difficult. We demonstrate a new methodology for diagnosing ozone production based on the processing of bonds contained within emitted molecules, the fate of which is determined by the conservation of spin of the bonding electrons. Using this methodology to diagnose ozone production in the GEOS-Chem chemical transport model, we demonstrate its advantages over the standard diagnostic. We show that the number of bonds emitted, their chemistry and lifetime, and feedbacks on OH are all important in determining the ozone production within the model and its sensitivity to changes. This insight may allow future model–model comparisons to better identify the root causes of model differences.

  4. Inclusion of inhomogeneous deformation and strength characteristics in the problem on zonal disintegration of rocks

    Science.gov (United States)

    Chanyshev, AI; Belousova, OE

    2018-03-01

    The authors determine stress and deformation in a heterogeneous rock mass at the preset displacement and Cauchy stress vector at the boundary of an underground excavation. The influence of coordinates on Young’s modulus, shear modulus and ultimate strength is shown. It is found that regions of tension and compression alternate at the excavation boundary—i.e. zonal rock disintegration phenomenon is observed.

  5. Boundary layers affected by different pressure gradients investigated computationally by a zonal RANS-LES method

    International Nuclear Information System (INIS)

    Roidl, B.; Meinke, M.; Schröder, W.

    2014-01-01

    Highlights: • Reformulated synthetic turbulence generation method (RSTGM) is applied. • Zonal RANS-LES method is applied to boundary layers at pressure gradients. • Good agreement with the pure LES and other reference data is obtained. • The RSTGM is applicable to pressure gradient flows without modification. • RANS-to-LES boundary should be located where -1·10 6 6 is satisfied. -- Abstract: The reformulated synthetic turbulence generation (RSTG) method is used to compute by a fully coupled zonal RANS-LES approach turbulent non-zero-pressure gradient boundary layers. The quality of the RSTG method, which is based on the same shape functions and length scale distributions as in zero-pressure gradient flow, is discussed by comparing the zonal RANS-LES findings with pure LES, pure RANS, direct numerical simulation (DNS), and experimental data. For the favorable pressure gradient (FPG) simulation the RANS-to-LES transition occurs in the accelerated flow region and for the adverse pressure gradient (APG) case it is located in the decelerated flow region. The results of the time and spanwise averaged skin-friction distributions, velocity profiles, and Reynolds stress distributions of the zonal RANS-LES simulation show a satisfactory to good agreement with the pure LES, reference DNS, and experimental data. The quality of the findings shows that the rigorous formulation of the synthetic turbulence generation makes the RSTG method applicable without a priori knowledge of the flow properties but those determined by the RANS solution and without using additional control planes to regulate the shear stress budget to a wide range of Reynolds numbers and pressure gradients. The method is a promising approach to formulate embedded RANS-to-LES boundaries in flow regions where the Pohlhausen or acceleration parameter satisfies -1·10 -6 ⩽K⩽2·10 -6

  6. A theory of self-organized zonal flow with fine radial structure in tokamak

    Science.gov (United States)

    Zhang, Y. Z.; Liu, Z. Y.; Xie, T.; Mahajan, S. M.; Liu, J.

    2017-12-01

    The (low frequency) zonal flow-ion temperature gradient (ITG) wave system, constructed on Braginskii's fluid model in tokamak, is shown to be a reaction-diffusion-advection system; it is derived by making use of a multiple spatiotemporal scale technique and two-dimensional (2D) ballooning theory. For real regular group velocities of ITG waves, two distinct temporal processes, sharing a very similar meso-scale radial structure, are identified in the nonlinear self-organized stage. The stationary and quasi-stationary structures reflect a particular feature of the poloidal group velocity. The equation set posed to be an initial value problem is numerically solved for JET low mode parameters; the results are presented in several figures and two movies that show the spatiotemporal evolutions as well as the spectrum analysis—frequency-wave number spectrum, auto power spectrum, and Lissajous diagram. This approach reveals that the zonal flow in tokamak is a local traveling wave. For the quasi-stationary process, the cycle of ITG wave energy is composed of two consecutive phases in distinct spatiotemporal structures: a pair of Cavitons growing and breathing slowly without long range propagation, followed by a sudden decay into many Instantons that carry negative wave energy rapidly into infinity. A spotlight onto the motion of Instantons for a given radial position reproduces a Blob-Hole temporal structure; the occurrence as well as the rapid decay of Caviton into Instantons is triggered by zero-crossing of radial group velocity. A sample of the radial profile of zonal flow contributed from 31 nonlinearly coupled rational surfaces near plasma edge is found to be very similar to that observed in the JET Ohmic phase [J. C. Hillesheim et al., Phys. Rev. Lett. 116, 165002 (2016)]. The theory predicts an interior asymmetric dipole structure associated with the zonal flow that is driven by the gradients of ITG turbulence intensity.

  7. The effect of the equatorially symmetric zonal winds of Saturn on its gravitational field

    Science.gov (United States)

    Kong, Dali; Zhang, Keke; Schubert, Gerald; Anderson, John D.

    2018-04-01

    The penetration depth of Saturn’s cloud-level winds into its interior is unknown. A possible way of estimating the depth is through measurement of the effect of the winds on the planet’s gravitational field. We use a self-consistent perturbation approach to study how the equatorially symmetric zonal winds of Saturn contribute to its gravitational field. An important advantage of this approach is that the variation of its gravitational field solely caused by the winds can be isolated and identified because the leading-order problem accounts exactly for rotational distortion, thereby determining the irregular shape and internal structure of the hydrostatic Saturn. We assume that (i) the zonal winds are maintained by thermal convection in the form of non-axisymmetric columnar rolls and (ii) the internal structure of the winds, because of the Taylor-Proundman theorem, can be uniquely determined by the observed cloud-level winds. We calculate both the variation ΔJn , n = 2, 4, 6 … of the axisymmetric gravitational coefficients Jn caused by the zonal winds and the non-axisymmetric gravitational coefficients ΔJnm produced by the columnar rolls, where m is the azimuthal wavenumber of the rolls. We consider three different cases characterized by the penetration depth 0.36, R S, 0.2, R S and 0.1, R S, where R S is the equatorial radius of Saturn at the 1-bar pressure level. We find that the high-degree gravitational coefficient (J 12 + ΔJ 12) is dominated, in all the three cases, by the effect of the zonal flow with |ΔJ 12/J 12| > 100% and that the size of the non-axisymmetric coefficients ΔJ mn directly reflects the depth and scale of the flow taking place in the Saturnian interior.

  8. Biomimetic multidirectional scaffolds for zonal osteochondral tissue engineering via a lyophilization bonding approach.

    Science.gov (United States)

    Clearfield, Drew; Nguyen, Andrew; Wei, Mei

    2018-04-01

    The zonal organization of osteochondral tissue underlies its long term function. Despite this, tissue engineering strategies targeted for osteochondral repair commonly rely on the use of isotropic biomaterials for tissue reconstruction. There exists a need for a new class of highly biomimetic, anisotropic scaffolds that may allow for the engineering of new tissue with zonal properties. To address this need, we report the facile production of monolithic multidirectional collagen-based scaffolds that recapitulate the zonal structure and composition of osteochondral tissue. First, superficial and osseous zone-mimicking scaffolds were fabricated by unidirectional freeze casting collagen-hyaluronic acid and collagen-hydroxyapatite-containing suspensions, respectively. Following their production, a lyophilization bonding process was used to conjoin these scaffolds with a distinct collagen-hyaluronic acid suspension mimicking the composition of the transition zone. Resulting matrices contained a thin, highly aligned superficial zone that interfaced with a cellular transition zone and vertically oriented calcified cartilage and osseous zones. Confocal microscopy confirmed a zone-specific localization of hyaluronic acid, reflecting the depth-dependent increase of glycosaminoglycans in the native tissue. Poorly crystalline, carbonated hydroxyapatite was localized to the calcified cartilage and osseous zones and bordered the transition zone. Compressive testing of hydrated scaffold zones confirmed an increase of stiffness with scaffold depth, where compressive moduli of chondral and osseous zones fell within or near ranges conducive for chondrogenesis or osteogenesis of mesenchymal stem cells. With the combination of these biomimetic architectural and compositional cues, these multidirectional scaffolds hold great promise for the engineering of zonal osteochondral tissue. © 2017 Wiley Periodicals, Inc. J Biomed Mater Res Part A: 106A: 948-958, 2018. © 2017 Wiley Periodicals

  9. Sensitivity of stomatal conductance to soil moisture: implications for tropospheric ozone

    Directory of Open Access Journals (Sweden)

    A. Anav

    2018-04-01

    Full Text Available Soil moisture and water stress play a pivotal role in regulating stomatal behaviour of plants; however, in the last decade, the role of water availability has often been neglected in atmospheric chemistry modelling studies as well as in integrated risk assessments, despite the fact that plants remove a large amount of atmospheric compounds from the lower troposphere through stomata. The main aim of this study is to evaluate, within the chemistry transport model CHIMERE, the effect of soil water limitation on stomatal conductance and assess the resulting changes in atmospheric chemistry testing various hypotheses of water uptake by plants in the rooting zone. Results highlight how dry deposition significantly declines when soil moisture is used to regulate the stomatal opening, mainly in the semi-arid environments: in particular, over Europe the amount of ozone removed by dry deposition in one year without considering any soil water limitation to stomatal conductance is about 8.5 TgO3, while using a dynamic layer that ensures that plants maximize the water uptake from soil, we found a reduction of about 10 % in the amount of ozone removed by dry deposition ( ∼  7.7 TgO3. Although dry deposition occurs from the top of canopy to ground level, it affects the concentration of gases remaining in the lower atmosphere, with a significant impact on ozone concentration (up to 4 ppb extending from the surface to the upper troposphere (up to 650 hPa. Our results shed light on the importance of improving the parameterizations of processes occurring at plant level (i.e. from the soil to the canopy as they have significant implications for concentration of gases in the lower troposphere and resulting risk assessments for vegetation or human health.

  10. Tropospheric weather influenced by solar wind through atmospheric vertical coupling downward control

    Science.gov (United States)

    Prikryl, Paul; Bruntz, Robert; Tsukijihara, Takumi; Iwao, Koki; Muldrew, Donald B.; Rušin, Vojto; Rybanský, Milan; Turňa, Maroš; Šťastný, Pavel

    2018-06-01

    Occurrence of severe weather in the context of solar wind coupling to the magnetosphere-ionosphere-atmosphere (MIA) system is investigated. It is observed that significant snowfall, wind and heavy rain, particularly if caused by low pressure systems in winter, tend to follow arrivals of high-speed solar wind. Previously published statistical evidence that explosive extratropical cyclones in the northern hemisphere tend to occur within a few days after arrivals of high-speed solar wind streams from coronal holes (Prikryl et al., 2009, 2016) is corroborated for the southern hemisphere. Cases of severe weather events are examined in the context of the magnetosphere-ionosphere-atmosphere (MIA) coupling. Physical mechanism to explain these observations is proposed. The leading edge of high-speed solar wind streams is a locus of large-amplitude magneto-hydrodynamic waves that modulate Joule heating and/or Lorentz forcing of the high-latitude lower thermosphere generating medium-scale atmospheric gravity waves that propagate upward and downward through the atmosphere. Simulations of gravity wave propagation in a model atmosphere using the Transfer Function Model (Mayr et al., 1990) reveal that propagating waves originating in the lower thermosphere can excite a spectrum of gravity waves in the lower atmosphere. In spite of significantly reduced amplitudes but subject to amplification upon reflection in the upper troposphere, these gravity waves can provide a lift of unstable air to release instabilities in the troposphere and initiate convection to form cloud/precipitation bands. It is primarily the energy provided by release of latent heat that leads to intensification of storms. These results indicate that vertical coupling in the atmosphere exerts downward control from solar wind to the lower atmospheric levels influencing tropospheric weather development.

  11. Sensitivity of stomatal conductance to soil moisture: implications for tropospheric ozone

    Science.gov (United States)

    Anav, Alessandro; Proietti, Chiara; Menut, Laurent; Carnicelli, Stefano; De Marco, Alessandra; Paoletti, Elena

    2018-04-01

    Soil moisture and water stress play a pivotal role in regulating stomatal behaviour of plants; however, in the last decade, the role of water availability has often been neglected in atmospheric chemistry modelling studies as well as in integrated risk assessments, despite the fact that plants remove a large amount of atmospheric compounds from the lower troposphere through stomata. The main aim of this study is to evaluate, within the chemistry transport model CHIMERE, the effect of soil water limitation on stomatal conductance and assess the resulting changes in atmospheric chemistry testing various hypotheses of water uptake by plants in the rooting zone. Results highlight how dry deposition significantly declines when soil moisture is used to regulate the stomatal opening, mainly in the semi-arid environments: in particular, over Europe the amount of ozone removed by dry deposition in one year without considering any soil water limitation to stomatal conductance is about 8.5 TgO3, while using a dynamic layer that ensures that plants maximize the water uptake from soil, we found a reduction of about 10 % in the amount of ozone removed by dry deposition ( ˜ 7.7 TgO3). Although dry deposition occurs from the top of canopy to ground level, it affects the concentration of gases remaining in the lower atmosphere, with a significant impact on ozone concentration (up to 4 ppb) extending from the surface to the upper troposphere (up to 650 hPa). Our results shed light on the importance of improving the parameterizations of processes occurring at plant level (i.e. from the soil to the canopy) as they have significant implications for concentration of gases in the lower troposphere and resulting risk assessments for vegetation or human health.

  12. Highly resolved global distribution of tropospheric NO2 using GOME narrow swath mode data

    Directory of Open Access Journals (Sweden)

    S. Beirle

    2004-01-01

    Full Text Available The Global Ozone Monitoring Experiment (GOME allows the retrieval of tropospheric vertical column densities (VCDs of NO2 on a global scale. Regions with enhanced industrial activity can clearly be detected, but the standard spatial resolution of the GOME ground pixels (320x40km2 is insufficient to resolve regional trace gas distributions or individual cities. Every 10 days within the nominal GOME operation, measurements are executed in the so called narrow swath mode with a much better spatial resolution (80x40km2. We use this data (1997-2001 to construct a detailed picture of the mean global tropospheric NO2 distribution. Since - due to the narrow swath - the global coverage of the high resolution observations is rather poor, it has proved to be essential to deseasonalize the single narrow swath mode observations to retrieve adequate mean maps. This is done by using the GOME backscan information. The retrieved high resolution map illustrates the shortcomings of the standard size GOME pixels and reveals an unprecedented wealth of details in the global distribution of tropospheric NO2. Localised spots of enhanced NO2 VCD can be directly associated to cities, heavy industry centers and even large power plants. Thus our result helps to check emission inventories. The small spatial extent of NO2 'hot spots' allows us to estimate an upper limit of the mean lifetime of boundary layer NOx of 17h on a global scale. The long time series of GOME data allows a quantitative comparison of the narrow swath mode data to the nominal resolution. Thus we can analyse the dependency of NO2 VCDs on pixel size. This is important for comparing GOME data to results of new satellite instruments like SCIAMACHY (launched March 2002 on ENVISAT, OMI (launched July 2004 on AURA or GOME II (to be launched 2005 with an improved spatial resolution.

  13. Analysis of equatorial plasma bubble zonal drift velocities in the Pacific sector by imaging techniques

    Directory of Open Access Journals (Sweden)

    D. Yao

    2007-03-01

    Full Text Available Using 1024 nights of data from 2002–2005 taken by the Cornell Narrow Field Imager (CNFI, we examine equatorial plasma bubble (EPB zonal drift velocity characteristics. CNFI is located at the Maui Space Surveillance Site on the Haleakala Volcano (geographic: 20.71° N, 203.83° E; geomagnetic: 21.03° N, 271.84° E on the island of Maui, Hawaii. The imager is set up to view in a magnetic field-aligned geometry in order to maximize its resolution. We calculate the zonal drift velocities using two methods: a correlation routine and an EPB west-wall intensity gradient tracking routine. These two methods yield sizeable differences in the evenings, suggesting strong pre-local midnight EPB development. An analysis of the drift velocities is also performed based on the three influencing factors of season, geomagnetic activity, and solar activity. In general, our data match published trends and drift characteristics from past studies. However, we find that the drift magnitudes are much lower than results from other imagers at similar latitude sectors but at different longitude sectors, suggesting that zonal drift velocities have a longitudinal dependence.

  14. MPIRUN: A Portable Loader for Multidisciplinary and Multi-Zonal Applications

    Science.gov (United States)

    Fineberg, Samuel A.; Woodrow, Thomas S. (Technical Monitor)

    1994-01-01

    Multidisciplinary and multi-zonal applications are an important class of applications in the area of Computational Aerosciences. In these codes, two or more distinct parallel programs or copies of a single program are utilized to model a single problem. To support such applications, it is common to use a programming model where a program is divided into several single program multiple data stream (SPMD) applications, each of which solves the equations for a single physical discipline or grid zone. These SPMD applications are then bound together to form a single multidisciplinary or multi-zonal program in which the constituent parts communicate via point-to-point message passing routines. One method for implementing the message passing portion of these codes is with the new Message Passing Interface (MPI) standard. Unfortunately, this standard only specifies the message passing portion of an application, but does not specify any portable mechanisms for loading an application. MPIRUN was developed to provide a portable means for loading MPI programs, and was specifically targeted at multidisciplinary and multi-zonal applications. Programs using MPIRUN for loading and MPI for message passing are then portable between all machines supported by MPIRUN. MPIRUN is currently implemented for the Intel iPSC/860, TMC CM5, IBM SP-1 and SP-2, Intel Paragon, and workstation clusters. Further, MPIRUN is designed to be simple enough to port easily to any system supporting MPI.

  15. Zonal Detached-Eddy Simulation of Turbulent Unsteady Flow over Iced Airfoils

    KAUST Repository

    Zhang, Yue

    2015-07-23

    This paper presentsamultiscale finite-element formulation for the second modeofzonal detached-eddy simulation. The multiscale formulation corrects the lack of stability of the standard Galerkin formulation by incorporating the effect of unresolved scales to the grid (resolved) scales. The stabilization terms arise naturally and are free of userdefined stability parameters. Validation of the method is accomplished via the turbulent flow over tandem cylinders. The boundary-layer separation, free shear-layer rollup, vortex shedding from the upstream cylinder, and interaction with the downstream cylinder are well reproduced. Good agreement with experimental measurements gives credence to the accuracy of zonal detached-eddy simulation in modeling turbulent separated flows. A comprehensive study is then conducted on the performance degradation of ice-contaminated airfoils. NACA 23012 airfoil with a spanwise ice ridge and Gates Learjet Corporation-305 airfoil with a leading-edge horn-shape glaze ice are selected for investigation. Appropriate spanwise domain size and sufficient grid density are determined to enhance the reliability of the simulations. A comparison of lift coefficient and flowfield variables demonstrates the added advantage that the zonal detached-eddy simulation model brings to the Spalart-Allmaras turbulence model. Spectral analysis and instantaneous visualization of turbulent structures are also highlighted via zonal detached-eddy simulation. Copyright © 2015 by the CFD Lab of McGill University. Published by the American Institute of Aeronautics and Astronautics, Inc.

  16. Multi-scale-nonlinear interactions among macro-MHD mode, micro-turbulence, and zonal flow

    International Nuclear Information System (INIS)

    Ishizawa, Akihiro; Nakajima, Noriyoshi

    2007-01-01

    This is the first numerical simulation demonstrating that macro-magnetohydrodynamic (macro-MHD) mode is exited as a result of multi-scale interaction in a quasi-steady equilibrium formed by a balance between zonal flow and micro-turbulence via reduced-two-fluid simulation. Only after obtaining the equilibrium which includes zonal flow and the turbulence caused by kinetic ballooning mode is this simulation of macro-MHD mode, double tearing mode, accomplished. In the quasi-steady equilibrium a macro-fluctuation which has the same helicity as that of double tearing mode is a part of the turbulence until it grows as a macro-MHD mode finally. When the macro-MHD grows it effectively utilize free energy of equilibrium current density gradient because of positive feedback loop between suppression of zonal flow and growth of the macro-fluctuation causing magnetic reconnection. Thus once the macro-MHD grows from the quasi-equilibrium, it does not go back. This simulation is more comparable with experimental observation of growing macro-fluctuation than traditional MHD simulation of linear instabilities in a static equilibrium. (author)

  17. Wind Diffusivity Current, QuikSCAT SeaWinds, 0.25 degrees, Global, Science Quality, Zonal

    Data.gov (United States)

    National Oceanic and Atmospheric Administration, Department of Commerce — NOAA CoastWatch distributes science quality Ekman current (in zonal, meridional, and modulus sets) and Ekman upwelling data. This data begins with wind velocity...

  18. TOMS EP UV Aerosol Index Daily and Monthly Zonal Means V008 (TOMSEPL3zaer) at GES DISC

    Data.gov (United States)

    National Aeronautics and Space Administration — This data product contains TOMS/EP UV Aerosol Index Daily and Monthly Zonal Means Version 8 data in ASCII format.The Total Ozone Mapping Spectrometer (TOMS) Version...

  19. Three-dimensional assembly of tissue-engineered cartilage constructs results in cartilaginous tissue formation without retainment of zonal characteristics

    NARCIS (Netherlands)

    Schuurman, W; Harimulyo, E B; Gawlitta, D; Woodfield, T B F; Dhert, Wouter J A; van Weeren, P. René; Malda, J

    Articular cartilage has limited regenerative capabilities. Chondrocytes from different layers of cartilage have specific properties, and regenerative approaches using zonal chondrocytes may yield better replication of the architecture of native cartilage than when using a single cell population. To

  20. Profiles of zonal flows and turbulence mode numbers and probe system in the HL-2A tokamak

    International Nuclear Information System (INIS)

    Hong Wenyu; Zhao Kaijun; Yan Longwen; Dong Jiaqi; Cheng Jun; Qian Jun

    2009-01-01

    The toroidal and poloidal symmetries (m-0, n-0) of the measured low frequency zonal flows (f=0-5 kHz) and geodesic acoustic mode zonal flow (f=16 kHz) electric potential and radial promulgate features were unambiguously identified with displaced Langmuir probe arrays in the edge plasma of the HL-2A tokamak for the first time. The finite radial wave vector (K r-LF =0.6 cm -1 , K r-GAM =2 cm -1 ) of the flows was simultaneously estimated. The formation mechanism of the flows is identified to be nonlinear three wave coupling between high frequency turbulent fluctuations and the flows. Changes of zonal flow amplitude bring by ECRH power and the boundary safety factors were simply studied. Moreover, change of zonal flow amplitude in radial direction was too observed. (authors)

  1. Measurements of upper atmosphere water vapor made in situ with a new moisture sensor

    Science.gov (United States)

    Chleck, D.

    1979-01-01

    A new thin-film aluminum oxide sensor, Aquamax II, has been developed for the measurement of stratospheric and upper tropospheric water vapor levels. The sensor is briefly described with attention given to its calibration and performance. Data obtained from six balloon flights are presented; almost all the results show a constant water vapor mixing ratio, in agreement with other data from midlatitude regions.

  2. CALL FOR PAPERS: Special cluster issue on `Experimental studies of zonal flow and turbulence'

    Science.gov (United States)

    Itoh, S.-I.

    2005-07-01

    Plasma Physics and Controlled Fusion (PPCF) invites submissions on the topic of `Experimental studies of zonal flow and turbulence', for consideration for a special topical cluster of articles to be published early in 2006. The topical cluster will be published in an issue of PPCF, combined with regular articles. The Guest Editor for the special cluster will be S-I Itoh, Kyushu University, Japan. There has been remarkable progress in the area of structure formation by turbulence. One of the highlights has been the physics of zonal flow and drift wave turbulence in toroidal plasmas. Extensive theoretical as well as computational studies have revealed the various mechanisms in turbulence and zonal flows. At the same time, experimental research on the zonal flow, geodesic acoustic modes and generation of global electric field by turbulence has evolved rapidly. Fast growth in reports of experimental results has stimulated further efforts to develop increased knowledge and systematic understanding. Each paper considered for the special cluster should describe the present research status and new scientific knowledge/results from the authors on experimental studies of zonal flow, geodesic acoustic modes and generation of electric field by turbulence (including studies of Reynolds-Maxwell stresses, etc). Manuscripts submitted to this special cluster in Plasma Physics and Controlled Fusion will be refereed according to the normal criteria and procedures of the journal. The Guest Editor guides the progress of the cluster from the initial open call, through the standard refereeing process, to publication. To be considered for inclusion in the special cluster, articles must be submitted by 2 September 2005 and must clearly state `for inclusion in the Turbulent Plasma Cluster'. Articles submitted after this deadline may not be included in the cluster issue but may be published in a later issue of the journal. Please submit your manuscript electronically via our web site at www

  3. Predicting temperature and moisture distributions in conditioned spaces using the zonal approach

    Energy Technology Data Exchange (ETDEWEB)

    Mendonca, K.C. [Parana Pontifical Catholic Univ., Curitiba (Brazil); Wurtz, E.; Inard, C. [La Rochelle Univ., La Rochelle, Cedex (France). LEPTAB

    2005-07-01

    Moisture interacts with building elements in a number of different ways that impact upon building performance, causing deterioration of building materials, as well as contributing to poor indoor air quality. In humid climates, moisture represents one of the major loads in conditioned spaces. It is therefore important to understand and model moisture transport accurately. This paper discussed an intermediate zonal approach to building a library of data in order to predict whole hygrothermal behavior in conditioned rooms. The zonal library included 2 models in order to consider building envelope moisture buffering effects as well as taking into account the dynamic aspect of jet airflow in the zonal method. The zonal library was then applied to a case study to show the impact of external humidity on the whole hygrothermal performance of a room equipped with a vertical fan-coil unit. The proposed theory was structured into 3 groups representing 3 building domains: indoor air; envelope; and heating, ventilation and air conditioning (HVAC) systems. The indoor air sub-model related to indoor air space, where airflow speed was considered to be low. The envelope sub-model related to the radiation exchanges between the envelope and its environment as well as to the heat and mass transfers through the envelope material. The HVAC system sub-model referred to the whole system including equipment, control and specific airflow from the equipment. All the models were coupled into SPARK, where the resulting set of non-linear equations were solved simultaneously. A case study of a large office conditioned by a vertical fan-coil unit with a rectangular air supply diffuser was presented. Details of the building's external and internal environment were provided, as well as convective heat and mass transfer coefficients and temperature distributions versus time. Results of the study indicated that understanding building material moisture buffering effects is as important as

  4. Tropospheric ozone and its precursors from the urban to the global scale from air quality to short-lived climate forcer

    Science.gov (United States)

    Monks, P. S.; Archibald, A. T.; Colette, A.; Cooper, O.; Coyle, M.; Derwent, R.; Fowler, D.; Granier, C.; Law, K. S.; Mills, G. E.; Stevenson, D. S.; Tarasova, O.; Thouret, V.; von Schneidemesser, E.; Sommariva, R.; Wild, O.; Williams, M. L.

    2015-08-01

    Ozone holds a certain fascination in atmospheric science. It is ubiquitous in the atmosphere, central to tropospheric oxidation chemistry, yet harmful to human and ecosystem health as well as being an important greenhouse gas. It is not emitted into the atmosphere but is a byproduct of the very oxidation chemistry it largely initiates. Much effort is focused on the reduction of surface levels of ozone owing to its health and vegetation impacts, but recent efforts to achieve reductions in exposure at a country scale have proved difficult to achieve owing to increases in background ozone at the zonal hemispheric scale. There is also a growing realisation that the role of ozone as a short-lived climate pollutant could be important in integrated air quality climate change mitigation. This review examines current understanding of the processes regulating tropospheric ozone at global to local scales from both measurements and models. It takes the view that knowledge across the scales is important for dealing with air quality and climate change in a synergistic manner. The review shows that there remain a number of clear challenges for ozone such as explaining surface trends, incorporating new chemical understanding, ozone-climate coupling, and a better assessment of impacts. There is a clear and present need to treat ozone across the range of scales, a transboundary issue, but with an emphasis on the hemispheric scales. New observational opportunities are offered both by satellites and small sensors that bridge the scales.

  5. Acetone in theGlobal Troposphere: Its Possible Role as a Global Source of PAN

    Science.gov (United States)

    Singh, H. B.; Kanakidou, M.

    1994-01-01

    Oxygenated hydrocarbons are thought to be important components of the atmosphere but, with the exception of formaldehyde, very little about their distribution and fate is known. Aircraft measurements of acetone (CH3COCH3), PAN (CH3CO3NO2) and other organic species (e. g. acetaldehyde, methanol and ethanol) have been performed over the Pacific, the southern Atlantic, and the subarctic atmospheres. Sampled areas extended from 0 to 12 km altitude over latitudes of 70 deg N to 40 deg S. All measurements are based on real time in-situ analysis of cryogenically preconcentrated air samples. Substantial concentrations of these oxygenated species (10-2000 ppt) have been observed at all altitudes and geographical locations in the troposphere. Important sources include, emissions from biomass burning, plant and vegetation, secondary oxidation of primary non-methane hydrocarbons, and man-made emissions. Direct measurements within smoke plumes have been used to estimate the biomass burning source. Photochemistry studies are used to suggest that acetone could provide a major source of peroxyacetyl radicals in the atmosphere and play an important role in sequestering reactive nitrogen. Model calculations show that acetone photolysis contributes significantly to PAN formation in the middle and upper troposphere.

  6. Thermal structure of the TTL and its relation to stratospheric-tropospheric exchange of water.

    Science.gov (United States)

    de La Torre Juárez, M.; Ao, C. O.; Schr\\O der, T. M.; Hermann, R.

    2004-12-01

    The annual cycle of the TTL fine scale thermal structure is described as captured by GPS radio occultation and the pressure levels of the ECMWF weather analysis. This annual cycle is compared to the annual cycle in water concentrations at the upper troposphere/lower stratosphere measured by HALOE. It is found that the saturation mixing ratios at the Cold Point Tropopause temperatures are consistent and sligthly below HALOE values with some temporal lag. This suggests that if dehydration mechanisms other than those associated with slow vertical asscent are working effectively, they must be counterbalanced by other hydration mechanisms. A comparison between saturation mixing ratios at the temperatures captured by GPS radio occultation and HALOE concentrations of water vapor show an annual cycle dominated by supersaturation in the boreal winter months, when the upward mass fluxes are larger, and subsaturation in the summer. The longitudinal dependence of these cycles is discussed and so is its possible implication for the seasonality of statospheric-tropospheric exchange of water.

  7. Changes in equatorial zonal circulations and precipitation in the context of the global warming and natural modes

    Science.gov (United States)

    Kim, B. H.; Ha, K. J.

    2017-12-01

    The strengthening and westward shift of Pacific Walker Circulation (PWC) is observed during the recent decades. However, the relative roles of global warming and natural variability on the change in PWC unclearly remain. By conducting numerical atmospheric general circulation model (AGCM) experiments using the spatial SST patterns in the global warming and natural modes which are obtained by the multi-variate EOF analysis from three variables including precipitation, sea surface temperature (SST), and divergent zonal wind, we indicated that the westward shift and strengthening of PWC are caused by the global warming SST pattern in the global warming mode and the negative Interdecadal Pacific Oscillation-like SST pattern in the natural mode. The SST distribution of the Pacific Ocean (PO) has more influence on the changes in equatorial zonal circulations and tropical precipitation than that of the Indian Ocean (IO) and Atlantic Ocean (AO). The change in precipitation is also related to the equatorial zonal circulations variation through the upward and downward motions of the circulations. The IO and AO SST anomalies in the global warming mode can affect on the changes in equatorial zonal circulations, but the influence of PO SST disturbs the Indian Walker circulation and Atlantic Walker circulation changes by the IO and AO. The zonal shift of PWC is found to be highly associated with a zonal gradient of SST over the PO through the idealized numerical AGCM experiments and predictions of CMIP5 models.

  8. Pulmonary microRNA profiling: implications in upper lobe predominant lung disease

    OpenAIRE

    Armstrong, David A.; Nymon, Amanda B.; Ringelberg, Carol S.; Lesseur, Corina; Hazlett, Haley F.; Howard, Louisa; Marsit, Carmen J.; Ashare, Alix

    2017-01-01

    Background Numerous pulmonary diseases manifest with upper lobe predominance including cystic fibrosis, smoking-related chronic obstructive pulmonary disease, and tuberculosis. Zonal hypoxia, characteristic of these pulmonary maladies, and oxygen stress in general is known to exert profound effects on various important aspects of cell biology. Lung macrophages are major participants in the pulmonary innate immune response and regional differences in macrophage responsiveness to hypoxia may co...

  9. Performance analysis of NOAA tropospheric signal delay model

    International Nuclear Information System (INIS)

    Ibrahim, Hassan E; El-Rabbany, Ahmed

    2011-01-01

    Tropospheric delay is one of the dominant global positioning system (GPS) errors, which degrades the positioning accuracy. Recent development in tropospheric modeling relies on implementation of more accurate numerical weather prediction (NWP) models. In North America one of the NWP-based tropospheric correction models is the NOAA Tropospheric Signal Delay Model (NOAATrop), which was developed by the US National Oceanic and Atmospheric Administration (NOAA). Because of its potential to improve the GPS positioning accuracy, the NOAATrop model became the focus of many researchers. In this paper, we analyzed the performance of the NOAATrop model and examined its effect on ionosphere-free-based precise point positioning (PPP) solution. We generated 3 year long tropospheric zenith total delay (ZTD) data series for the NOAATrop model, Hopfield model, and the International GNSS Services (IGS) final tropospheric correction product, respectively. These data sets were generated at ten IGS reference stations spanning Canada and the United States. We analyzed the NOAATrop ZTD data series and compared them with those of the Hopfield model. The IGS final tropospheric product was used as a reference. The analysis shows that the performance of the NOAATrop model is a function of both season (time of the year) and geographical location. However, its performance was superior to the Hopfield model in all cases. We further investigated the effect of implementing the NOAATrop model on the ionosphere-free-based PPP solution convergence and accuracy. It is shown that the use of the NOAATrop model improved the PPP solution convergence by 1%, 10% and 15% for the latitude, longitude and height components, respectively

  10. Free-tropospheric BrO investigations based on GOME

    Science.gov (United States)

    Post, P.; van Roozendael, M.; Backman, L.; Damski, J.; Thölix, L.; Fayt, C.; Taalas, P.

    2003-04-01

    Bromine compounds contribute significantly to the stratospheric ozone depletion. However measurements of most bromine compounds are sparse or non-existent, and experimental studies essentially rely on BrO observations. The differences between balloon and ground based measurements of stratospheric BrO columns and satellite total column measurements are too large to be explained by measurement uncertainties. Therefore, it has been assumed that there is a concentration of BrO in the free troposphere of about 1-3 ppt. In a previous work, we have calculated the tropospheric BrO abundance as the difference between total BrO and stratospheric BrO columns. The total vertical column densities of BrO are extracted from GOME measurements using IASB-BIRA algorithms. The stratospheric amount has been calculated using chemical transport models (CTM). Results from SLIMCAT and FinROSE simulations are used for this purpose. SLIMCAT is a widely used 3D CTM that has been tested against balloon measurements. FinROSE is a 3D CTM developed at FMI. We have tried several different tropospheric BrO profiles. Our results show that a profile with high BrO concentrations in the boundary layer usually gives unrealistically high tropospheric column values over areas of low albedo (like oceans). This suggests that the tropospheric BrO would be predominantly distributed in the free troposphere. In this work, attempts are made to identify the signature of a free tropospheric BrO content when comparing cloudy and non-cloudy scenes. The possible impact of orography on measured BrO columns is also investigated.

  11. An assessment of 10-year NOAA aircraft-based tropospheric ozone profiling in Colorado

    Science.gov (United States)

    Leonard, Mark; Petropavlovskikh, Irina; Lin, Meiyun; McClure-Begley, Audra; Johnson, Bryan J.; Oltmans, Samuel J.; Tarasick, David

    2017-06-01

    The Global Greenhouse Gas Reference Network Aircraft Program at NOAA has sampled ozone and other atmospheric trace constituents in North America for over a decade (2005-present). The method to derive tropospheric ozone climatology from the light aircraft measurements equipped with the 2B Technology instruments is described in this paper. Since ozone instruments at most of aircraft locations are flown once a month, this raises the question of whether the sampling frequency allows for deriving a climatology that can adequately represent ozone seasonal and vertical variability over various locations. Here we interpret the representativeness of the tropospheric ozone climatology derived from these under-sampled observations using hindcast simulations conducted with the Geophysical Fluid Dynamics Laboratory chemistry-climate model (GFDL-AM3). We first focus on ozone measurements from monthly aircraft profiles over the Front Range of Colorado and weekly ozonesondes launched in Boulder, Colorado. The climatology is presented as monthly values separated in 5th, 25th, 50th, 75th, 95th percentiles, and averaged at three vertical layers: lower (1.6-3 km), middle (3-6 km), and upper (6-8 km) troposphere. The aircraft-based climatology is compared to the climatology derived from the nearest located ozonesondes launched from Boulder, Colorado, from GFDL-AM3 co-sampled in time with in-situ observations, and from GFDL-AM3 continuous 3-h samples. Based on these analyses, we recommend the sampling frequency to obtain adequate representation of ozone climatology in the free troposphere. The 3-h sampled AM3 model is used as a benchmark reference for the under-sampled time series. We find that the minimal number of soundings required per month for the all altitude bins (1.6-3, 3-6, and 6-8 km) to sufficiently match the 95% confidence level of the fully sampled monthly ozone means vary between 3 and 5 sounding per month, except in August with a minimum of 6 soundings per month. The

  12. Influence of the North Atlantic Oscillation on European tropospheric composition: an observational and modelling study

    Science.gov (United States)

    Pope, R.; Chipperfield, M.

    2017-12-01

    The North Atlantic Oscillation (NAO) has a strong influence on winter-time North Atlantic and European circulation patterns. Under the positive phase of the NAO (NAO+), intensification of the climatological Icelandic low and Azores high pressure systems results in strong westerly flow across the Atlantic into Europe. Under the NAO negative phase (NAO-), there is a weakening of this meridional pressure gradient resulting in a southerly shift in the westerlies flow towards the sub-tropical Atlantic. Therefore, NAO+ and NAO- introduce unstable stormy and drier stable conditions into Europe, respectively. Under NAO+ conditions, the strong westerlies tend to enhance transport of European pollution (e.g. nitrogen oxides) away from anthropogenic source regions. While during NAO-, the more stable conditions lead to a build up of pollutants. However, secondary pollutants (i.e. tropospheric ozone) show the opposite signal where NAO+, while transporting primary pollutants away, introduces Atlantic ozone enriched air into Europe. Here ozone can form downwind of pollution from continental North America and be transported into Europe via the westerly flow. Under NAO-, this westerly ozone transport is reduced yielding lower European ozone concentrations also depleted further by ozone loss through the reaction with NOx, which has accumulated over the continent. Peroxyacetyl nitrate (PAN), observed in the upper troposphere - lower stratosphere (UTLS) by satellite, peaks over Iceland/Southern Greenland in NAO-, between 200-100 hPa, consistent with trapping by an anticyclone at this altitude. During NAO+, PAN is enhanced over the sub-tropical Atlantic and Arctic. Model simulations show that enhanced PAN over Iceland/Southern Greenland in NAO- is associated with vertical transport from the troposphere into the UTLS, while peak Arctic PAN in NAO+ is its accumulation given the strong northerly meridional transport in the UTLS. UTLS ozone spatial anomalies, relative to the winter

  13. Impact of a simple parameterization of convective gravity-wave drag in a stratosphere-troposphere general circulation model and its sensitivity to vertical resolution

    Directory of Open Access Journals (Sweden)

    C. Bossuet

    Full Text Available Systematic westerly biases in the southern hemisphere wintertime flow and easterly equatorial biases are experienced in the Météo-France climate model. These biases are found to be much reduced when a simple parameterization is introduced to take into account the vertical momentum transfer through the gravity waves excited by deep convection. These waves are quasi-stationary in the frame of reference moving with convection and they propagate vertically to higher levels in the atmosphere, where they may exert a significant deceleration of the mean flow at levels where dissipation occurs. Sixty-day experiments have been performed from a multiyear simulation with the standard 31 levels for a summer and a winter month, and with a T42 horizontal resolution. The impact of this parameterization on the integration of the model is found to be generally positive, with a significant deceleration in the westerly stratospheric jet and with a reduction of the easterly equatorial bias. The sensitivity of the Météo-France climate model to vertical resolution is also investigated by increasing the number of vertical levels, without moving the top of the model. The vertical resolution is increased up to 41 levels, using two kinds of level distribution. For the first, the increase in vertical resolution concerns especially the troposphere (with 22 levels in the troposphere, and the second treats the whole atmosphere in a homogeneous way (with 15 levels in the troposphere; the standard version of 31 levels has 10 levels in the troposphere. A comparison is made between the dynamical aspects of the simulations. The zonal wind and precipitation are presented and compared for each resolution. A positive impact is found with the finer tropospheric resolution on the precipitation in the mid-latitudes and on the westerly stratospheric jet, but the general impact on the model climate is weak, the physical parameterizations used appear to be mostly independent to the

  14. New capability for ozone dial profiling measurements in the troposphere and lower stratosphere from aircraft

    Science.gov (United States)

    Hair, Johnathan; Hostetler, Chris; Cook, Anthony; Harper, David; Notari, Anthony; Fenn, Marta; Newchurch, Mike; Wang, Lihua; Kuang, Shi; Knepp, Travis; Burton, Sharon; Ferrare, Richard; Butler, Carolyn; Collins, Jim; Nehrir, Amin

    2018-04-01

    Recently, we successfully demonstrated a new compact and robust ozone DIAL lidar for smaller aircraft such as the NASA B200 and the ER-2 high-altitude aircraft. This is the first NASA airborne lidar to incorporate advanced solid-state lasers to produce the required power at the required ultraviolet wavelengths, and is compact and robust enough to operate nearly autonomously on the high-altitude ER-2 aircraft. This technology development resulted in the first new NASA airborne ozone DIAL instrument in more than 15 years. The combined ozone, aerosol, and clouds measurements provide valuable information on the chemistry, radiation, and dynamics of the atmosphere. In particular, from the ER-2 it offers a unique capability to study the upper troposphere and lower stratosphere.

  15. On the effect of moisture on the detection of tropospheric turbulence from in situ measurements

    Directory of Open Access Journals (Sweden)

    R. Wilson

    2013-03-01

    Full Text Available The present paper addresses the detection of turbulence based on the Thorpe (1977 method applied to an atmosphere where saturation of water vapor occurs. The detection method proposed by Thorpe relies on the sorting in ascending order of a measured profile of a variable conserved through adiabatic processes, (e.g. potential temperature. For saturated air, the reordering should be applied to a moist-conservative potential temperature, θm, which is analogous to potential temperature for a dry (subsaturated atmosphere. Here, θm is estimated from the Brunt–Väisälä frequency derived by Lalas and Einaudi (1974 in a saturated atmosphere. The application to balloon data shows that the effective turbulent fraction of the troposphere can dramatically increase when saturation is taken into account. Preliminary results of comparisons with data simultaneously collected from the VHF Middle and Upper atmosphere radar (MUR, Japan seem to give credence to the proposed approach.

  16. New capability for ozone dial profiling measurements in the troposphere and lower stratosphere from aircraft

    Directory of Open Access Journals (Sweden)

    Hair Johnathan

    2018-01-01

    Full Text Available Recently, we successfully demonstrated a new compact and robust ozone DIAL lidar for smaller aircraft such as the NASA B200 and the ER-2 high-altitude aircraft. This is the first NASA airborne lidar to incorporate advanced solid-state lasers to produce the required power at the required ultraviolet wavelengths, and is compact and robust enough to operate nearly autonomously on the high-altitude ER-2 aircraft. This technology development resulted in the first new NASA airborne ozone DIAL instrument in more than 15 years. The combined ozone, aerosol, and clouds measurements provide valuable information on the chemistry, radiation, and dynamics of the atmosphere. In particular, from the ER-2 it offers a unique capability to study the upper troposphere and lower stratosphere.

  17. Carbon monoxide and methane in the North American Arctic and Subarctic troposphere - July-August 1988

    Energy Technology Data Exchange (ETDEWEB)

    Harriss, R.C.; Sachse, G.W.; Hill, G.F.; Wade, L.; Bartlett, K.B.; Collins, J.E.; Steele, L.P.; Novelli, P.C. (New Hampshire Univ., Durham (United States) NASA, Langley Research Center, Hampton, VA (United States) Lockheed Engineering Sciences Co., Hampton, VA (United States) Science and Technology Corp., Hampton, VA (United States) Cooperative Inst. for Research in Environmental Sciences, Boulder, CO (United States))

    1992-10-01

    Enhanced concentrations of CH4 in the unpolluted atmospheric mixed layer over both Arctic and subarctic tundra landscapes are documented here using data from the NASA Arctic Boundary Layer Expedition (ABLE 3A). The CH4 concentration gradients were determined mainly by interactions of biogenic emission from wet tundra and turbulent mixing proceses. The gradient were most frequently associated with intrusion of upper tropospheric or stratospheric air into the midtroposphere, emissions from forest and tundra fires, and long-range transport of enhanced concentration of these gases from unidentified sources. Summertime haze layers exhibited midtropospheric enhancements of CH4 similar to those measured in winter Arctic events. The observations confirm the importance of Arctic and Subarctic wetland environments as a regional source of global atmospheric CH4. 33 refs.

  18. Carbon monoxide and methane in the North American Arctic and Subarctic troposphere - July-August 1988

    Science.gov (United States)

    Harriss, Robert C.; Sachse, Glen W.; Hill, Gerald F.; Wade, Larry; Bartlett, Karen B.; Collins, James E.; Steele, L. P.; Novelli, Paul C.

    1992-01-01

    Enhanced concentrations of CH4 in the unpolluted atmospheric mixed layer over both Arctic and subarctic tundra landscapes are documented here using data from the NASA Arctic Boundary Layer Expedition (ABLE 3A). The CH4 concentration gradients were determined mainly by interactions of biogenic emission from wet tundra and turbulent mixing proceses. The gradient were most frequently associated with intrusion of upper tropospheric or stratospheric air into the midtroposphere, emissions from forest and tundra fires, and long-range transport of enhanced concentration of these gases from unidentified sources. Summertime haze layers exhibited midtropospheric enhancements of CH4 similar to those measured in winter Arctic events. The observations confirm the importance of Arctic and Subarctic wetland environments as a regional source of global atmospheric CH4.

  19. Applying Kalman filtering to investigate tropospheric effects in VLBI

    Science.gov (United States)

    Soja, Benedikt; Nilsson, Tobias; Karbon, Maria; Heinkelmann, Robert; Liu, Li; Lu, Cuixian; Andres Mora-Diaz, Julian; Raposo-Pulido, Virginia; Xu, Minghui; Schuh, Harald

    2014-05-01

    Very Long Baseline Interferometry (VLBI) currently provides results, e.g., estimates of the tropospheric delays, with a delay of more than two weeks. In the future, with the coming VLBI2010 Global Observing System (VGOS) and increased usage of electronic data transfer, it is planned that the time between observations and results is decreased. This may, for instance, allow the integration of VLBI-derived tropospheric delays into numerical weather prediction models. Therefore, future VLBI analysis software packages need to be able to process the observational data autonomously in near real-time. For this purpose, we have extended the Vienna VLBI Software (VieVS) by a Kalman filter module. This presentation describes the filter and discusses its application for tropospheric studies. Instead of estimating zenith wet delays as piece-wise linear functions in a least-squares adjustment, the Kalman filter allows for more sophisticated stochastic modeling. We start with a random walk process to model the time-dependent behavior of the zenith wet delays. Other possible approaches include the stochastic model described by turbulence theory, e.g. the model by Treuhaft and Lanyi (1987). Different variance-covariance matrices of the prediction error, depending on the time of the year and the geographic latitude, have been tested. In winter and closer to the poles, lower variances and covariances are appropriate. The horizontal variations in tropospheric delays have been investigated by comparing three different strategies: assumption of a horizontally stratified troposphere, using north and south gradients modeled, e.g., as Gauss-Markov processes, and applying a turbulence model assuming correlations between observations in different azimuths. By conducting Monte-Carlo simulations of current standard VLBI networks and of future VGOS networks, the different tropospheric modeling strategies are investigated. For this purpose, we use the simulator module of VieVS which takes into

  20. Impact of selected troposphere models on Precise Point Positioning convergence

    Science.gov (United States)

    Kalita, Jakub; Rzepecka, Zofia

    2016-04-01

    The Precise Point Positioning (PPP) absolute method is currently intensively investigated in order to reach fast convergence time. Among various sources that influence the convergence of the PPP, the tropospheric delay is one of the most important. Numerous models of tropospheric delay are developed and applied to PPP processing. However, with rare exceptions, the quality of those models does not allow fixing the zenith path delay tropospheric parameter, leaving difference between nominal and final value to the estimation process. Here we present comparison of several PPP result sets, each of which based on different troposphere model. The respective nominal values are adopted from models: VMF1, GPT2w, MOPS and ZERO-WET. The PPP solution admitted as reference is based on the final troposphere product from the International GNSS Service (IGS). The VMF1 mapping function was used for all processing variants in order to provide capability to compare impact of applied nominal values. The worst case initiates zenith wet delay with zero value (ZERO-WET). Impact from all possible models for tropospheric nominal values should fit inside both IGS and ZERO-WET border variants. The analysis is based on data from seven IGS stations located in mid-latitude European region from year 2014. For the purpose of this study several days with the most active troposphere were selected for each of the station. All the PPP solutions were determined using gLAB open-source software, with the Kalman filter implemented independently by the authors of this work. The processing was performed on 1 hour slices of observation data. In addition to the analysis of the output processing files, the presented study contains detailed analysis of the tropospheric conditions for the selected data. The overall results show that for the height component the VMF1 model outperforms GPT2w and MOPS by 35-40% and ZERO-WET variant by 150%. In most of the cases all solutions converge to the same values during first

  1. Tropospheric ozone observations - How well can we assess tropospheric ozone changes?

    Science.gov (United States)

    Tarasick, D. W.; Galbally, I. E.; Ancellet, G.; Leblanc, T.; Wallington, T. J.; Ziemke, J. R.; Steinbacher, M.; Stähelin, J.; Vigouroux, C.; Hannigan, J. W.; García, O. E.; Foret, G.; Zanis, P.; Liu, X.; Weatherhead, E. C.; Petropavlovskikh, I. V.; Worden, H. M.; Osman, M.; Liu, J.; Lin, M.; Cooper, O. R.; Schultz, M. G.; Granados-Muñoz, M. J.; Thompson, A. M.; Cuesta, J.; Dufour, G.; Thouret, V.; Hassler, B.; Trickl, T.

    2017-12-01

    Since the early 20th century, measurements of ozone in the free troposphere have evolved and changed. Data records have different uncertainties and biases, and differ with respect to coverage, information content, and representativeness. Almost all validation studies employ ECC ozonesondes. These have been compared to UV-absorption measurements in a number of intercomparison studies, and show a modest ( 1-5%) high bias in the troposphere, with an uncertainty of 5%, but no evidence of a change over time. Umkehr, lidar, FTIR, and commercial aircraft all show modest low biases relative to the ECCs, and so -- if the ECC biases are transferable -- all agree within 1σ with the modern UV standard. Relative to the UV standard, Brewer-Mast sondes show a 20% increase in sensitivity from 1970-1995, while Japanese KC sondes show an increase of 5-10%. Combined with the shift of the global ozonesonde network to ECCs, this can induce a false positive trend, in analyses based on sonde data. Passive sounding methods -- Umkehr, FTIR and satellites -- have much lower vertical resolution than active methods, and this can limit the attribution of trends. Satellite biases are larger than those of other measurement systems, ranging between -10% and +20%, and standard deviations are large: about 10-30%, versus 5-10% for sondes, aircraft, lidar and ground-based FTIR. There is currently little information on measurement drift for satellite measurements of tropospheric ozone. This is an evident area of concern if satellite retrievals are used for trend studies. The importance of ECC sondes as a transfer standard for satellite validation means that efforts to homogenize existing records, by correcting for known changes and by adopting strict standard operating procedures, should continue, and additional research effort should be put into understanding and reducing sonde uncertainties. Representativeness is also a potential source of large errors, which are difficult to quantify. The global

  2. Retrieval of tropospheric carbon monoxide for the MOPITT experiment

    Science.gov (United States)

    Pan, Liwen; Gille, John C.; Edwards, David P.; Bailey, Paul L.; Rodgers, Clive D.

    1998-12-01

    A retrieval method for deriving the tropospheric carbon monoxide (CO) profile and column amount under clear sky conditions has been developed for the Measurements of Pollution In The Troposphere (MOPITT) instrument, scheduled for launch in 1998 onboard the EOS-AM1 satellite. This paper presents a description of the method along with analyses of retrieval information content. These analyses characterize the forward measurement sensitivity, the contribution of a priori information, and the retrieval vertical resolution. Ensembles of tropospheric CO profiles were compiled both from aircraft in situ measurements and from chemical model results and were used in retrieval experiments to characterize the method and to study the sensitivity to different parameters. Linear error analyses were carried out in parallel with the ensemble experiments. Results of these experiments and analyses indicate that MOPITT CO column measurements will have better than 10% precision, and CO profile measurement will have approximately three pieces of independent information that will resolve 3-5 tropospheric layers to approximately 10% precision. These analyses are important for understanding MOPITT data, both for application of data in tropospheric chemistry studies and for comparison with in situ measurements.

  3. Sulfate Aerosols from Non-Explosive Volcanoes: Chemical-Radiative Effects in the Troposphere and Lower Stratosphere

    Directory of Open Access Journals (Sweden)

    Giovanni Pitari

    2016-06-01

    Full Text Available SO2 and H2S are the two most important gas-phase sulfur species emitted by volcanoes, with a global amount from non-explosive emissions of the order 10 Tg-S/yr. These gases are readily oxidized forming SO42− aerosols, which effectively scatter the incoming solar radiation and cool the surface. They also perturb atmospheric chemistry by enhancing the NOx to HNO3 heterogeneous conversion via hydrolysis on the aerosol surface of N2O5 and Br-Cl nitrates. This reduces formation of tropospheric O3 and the OH to HO2 ratio, thus limiting the oxidation of CH4 and increasing its lifetime. In addition to this tropospheric chemistry perturbation, there is also an impact on the NOx heterogeneous chemistry in the lower stratosphere, due to vertical transport of volcanic SO2 up to the tropical tropopause layer. Furthermore, the stratospheric O3 formation and loss, as well as the NOx budget, may be slightly affected by the additional amount of upward diffused solar radiation and consequent increase of photolysis rates. Two multi-decadal time-slice runs of a climate-chemistry-aerosol model have been designed for studying these chemical-radiative effects. A tropopause mean global net radiative flux change (RF of −0.23 W·m−2 is calculated (including direct and indirect aerosol effects with a 14% increase of the global mean sulfate aerosol optical depth. A 5–15 ppt NOx decrease is found in the mid-troposphere subtropics and mid-latitudes and also from pole to pole in the lower stratosphere. The tropospheric NOx perturbation triggers a column O3 decrease of 0.5–1.5 DU and a 1.1% increase of the CH4 lifetime. The surface cooling induced by solar radiation scattering by the volcanic aerosols induces a tropospheric stabilization with reduced updraft velocities that produce ice supersaturation conditions in the upper troposphere. A global mean 0.9% decrease of the cirrus ice optical depth is calculated with an indirect RF of −0.08 W·m−2.

  4. Monitoring the response of the upper troposphere/lower stratosphere to a greenhouse gas scenario

    International Nuclear Information System (INIS)

    Davis, J.M.; Cox, S.K.

    1992-01-01

    During the past two years a system has been under development to contribute to this monitoring process by making measurement of the downwelling infrared radiance field at moderate spectral resolution. Sensitivity of the measurements to the presence of cirrus cloudiness, and effective particle size in cirrus clouds has been demonstrated. Sensitivity of the measurements to concentration of C0 2 and to the gross temperature structure of a 2CO 2 atmosphere have been modeled, and measurements have been made at various locations to provide a data base for further system evaluation. A temperature retrieval algorithm has been acquired and examined concerning its potential for monitoring temperature and gaseous concentration profiles. A continue research program is described herein that may be divided into three parts. First, continued system development must be pursued. This includes continued attention to the absolute accuracy of the measurements, and implementation of the Path Characterization Algorithm (retrieval code). Second, the value of long term deployment of the system at a site of considerable elevation is necessary. Third, inclusion of a solar transmission capability at moderate resolution is proposed

  5. Diurnal variations of humidity and ice water content in the tropical upper troposphere

    Directory of Open Access Journals (Sweden)

    P. Eriksson

    2010-12-01

    Full Text Available Observational results of diurnal variations of humidity from Odin-SMR and AURA-MLS, and cloud ice mass from Odin-SMR and CloudSat are presented for the first time. Comparisons show that the retrievals of humidity and cloud ice from these two satellite combinations are in good agreement. The retrieved data are combined from four almost evenly distributed times of the day allowing mean values, amplitudes and phases of the diurnal variations around 200 hpa to be estimated. This analysis is applied to six climatologically distinct regions, five located in the tropics and one over the subtropical northern Pacific Ocean. The strongest diurnal cycles are found over tropical land regions, where the amplitude is ~7 RHi for humidity and ~50% for ice mass. The greatest ice mass for these regions is found during the afternoon, and the humidity maximum is observed to lag this peak by ~6 h. Over tropical ocean regions the variations are smaller and the maxima in both ice mass and humidity are found during the early morning. Observed results are compared with output from three climate models (ECHAM, EC-EARTH and CAM3. Direct measurement-model comparisons were not possible because the measured and modelled cloud ice masses represent different quantities. To make a meaningful comparison, the amount of snow had to be estimated from diagnostic parameters of the models. There is a high probability that the models underestimate the average ice mass (outside the 1-σ uncertainty. The models also show clear deficiencies when it comes to amplitude and phase of the regional variations, but to varying degrees.

  6. Upper atmosphere tidal oscillations due to latent heat release in the tropical troposphere

    Directory of Open Access Journals (Sweden)

    J. M. Forbes

    1997-09-01

    Full Text Available Latent heat release associated with tropical deep convective activity is investigated as a source for migrating (sun-synchronous diurnal and semidiurnal tidal oscillations in the 80–150-km height region. Satellite-based cloud brightness temperature measurements made between 1988 and 1994 and averaged into 3-h bins are used to determine the annual- and longitude-average local-time distribution of rainfall rate, and hence latent heating, between ±40° latitude. Regional average rainfall rates are shown to be in good agreement with climatological values derived from surface rain gauge data. A global linearized wave model is used to estimate the corresponding atmospheric perturbations in the mesosphere/lower thermosphere (80–150 km resulting from upward-propagating tidal components excited by the latent heating. The annual-average migrating diurnal and semidiurnal components achieve velocity and temperature amplitudes of order 10–20 m s–1 and 5–10 K, respectively, which represent substantial contributions to the dynamics of the region. The latent heat forcing also shifts the phase (local solar time of maximum of the semidiurnal surface pressure oscillation from 0912 to 0936 h, much closer to the observed value of 0944 h.

  7. Sources of HO x and production of ozone in the upper troposphere over the United States

    OpenAIRE

    Jaeglé, L.; Jacob, Daniel James; Brune, W. H.; Tan, D.; Faloona, I. C.; Weinheimer, A. J.; Ridley, B. A.; Campos, T. L.; Sachse, G. W.

    1998-01-01

    The sources of HOx (OH+peroxy radicals) and the associated production of ozone at 8–12 km over the United States are examined by modeling observations of OH, HO2, NO, and other species during the SUCCESS aircraft campaign in April–May 1996. The HOx concentrations measured in SUCCESS are up to a factor of 3 higher than can be calculated from oxidation of water vapor and photolysis of acetone. The highest discrepancy was seen in the outflow of a convective storm. We show that convective injecti...

  8. Monitoring the response of the upper troposphere/lower stratosphere to a greenhouse gas scenario

    International Nuclear Information System (INIS)

    Davis, J.M.; Cox, S.K.

    1991-01-01

    The emission interferometer system deployed at a high elevation site in the foothills of the Rocky Mountains. Spectra and atmospheric soundings were collected under various sky conditions. Spectra were collected at different observation zenith angles to investigate those portions of the spectrum most sensitive to changes in atmospheric path. The stability of the 60 degrees/O degrees radiance ratios have been evaluated for the small number of clear sky spectra collected to date. Initial results indicate that the ratio is constant to about 0.5% (excluding large variations in the temperature structure) for clear sky cases. The ratio also shows sensitivity even to thin cloudiness. Examination of the spectra in the atmospheric window region shows that the slope of the floor of the spectra is sensitive even to near sub-visual cirrus conditions. A temperature and gaseous concentration retrieval algorithm has been acquired to investigate the more conventional inversion to the current problem. A high speed computer workstation has been acquired to facilitate this phase of the research. 1 ref., 5 figs

  9. Transport of biomass burning smoke to the upper troposphere by deep convection in the equatorial region

    NARCIS (Netherlands)

    Andreae, M. O.; Artaxo, P.; Fischer, H.; Freitas, S. R.; Grégoire, J.-M.; Hansel, A.; Hoor, P.; Kormann, R.; Krejci, R.; Lange, L.; Lelieveld, J.; Lindinger, W.; Longo, K.; Peters, W.; de Reus, M.; Scheeren, B.; Silva Dias, M. A. F.; Ström, J.; van Velthoven, P. F. J.; Williams, J.

    2001-01-01

    During LBA-CLAIRE-98, we found atmospheric layers with aged biomass smoke at altitudes >10 km over Suriname. CO, CO2, acetonitrile, methyl chloride, hydrocarbons, NO, O3, and aerosols were strongly enhanced in these layers. We estimate that 80-95% of accumulation mode aerosols had been removed

  10. What controls the low ice number concentration in the upper troposphere?

    Directory of Open Access Journals (Sweden)

    C. Zhou

    2016-10-01

    Full Text Available Cirrus clouds in the tropical tropopause play a key role in regulating the moisture entering the stratosphere through their dehydrating effect. Low ice number concentrations ( <  200 L−1 and high supersaturations (150–160 % have been observed in these clouds. Different mechanisms have been proposed to explain these low ice number concentrations, including the inhibition of homogeneous freezing by the deposition of water vapour onto pre-existing ice crystals, heterogeneous ice formation on glassy organic aerosol ice nuclei (IN, and limiting the formation of ice number from high-frequency gravity waves. In this study, we examined the effect from three different representations of updraft velocities, the effect from pre-existing ice crystals, the effect from different water vapour deposition coefficients (α  =  0.1 or 1, and the effect of 0.1 % of the total secondary organic aerosol (SOA particles acting as IN. Model-simulated ice crystal numbers are compared against an aircraft observational dataset.Including the effect from water vapour deposition on pre-existing ice particles can effectively reduce simulated in-cloud ice number concentrations for all model setups. A larger water vapour deposition coefficient (α  =  1 can also efficiently reduce ice number concentrations at temperatures below 205 K, but less so at higher temperatures. SOA acting as IN is most effective at reducing ice number concentrations when the effective updraft velocities are moderate ( ∼  0.05–0.2 m s−1. However, the effects of including SOA as IN and using (α  =  1 are diminished when the effect from pre-existing ice is included.When a grid-resolved large-scale updraft velocity ( <  0.1 m s−1 is used, the ice nucleatio