Ultrafast optical control of terahertz surface plasmons in subwavelength hole-arrays at room temperature

Energy Technology Data Exchange (ETDEWEB)

Azad, Abul Kalam [Los Alamos National Laboratory; Chen, Hou - Tong [Los Alamos National Laboratory; Taylor, Antoinette [Los Alamos National Laboratory; O' Hara, John [Los Alamos National Laboratory

2010-12-10

Extraordinary optical transmission through subwavelength metallic hole-arrays has been an active research area since its first demonstration. The frequency selective resonance properties of subwavelength metallic hole arrays, generally known as surface plasmon polaritons, have potential use in functional plasmonic devices such as filters, modulators, switches, etc. Such plasmonic devices are also very promising for future terahertz applications. Ultrafast switching or modulation of the resonant behavior of the 2-D metallic arrays in terahertz frequencies is of particular interest for high speed communication and sensing applications. In this paper, we demonstrate optical control of surface plasmon enhanced resonant terahertz transmission in two-dimensional subwavelength metallic hole arrays fabricated on gallium arsenide based substrates. Optically pumping the arrays creates a conductive layer in the substrate reducing the terahertz transmission amplitude of both the resonant mode and the direct transmission. Under low optical fluence, the terahertz transmission is more greatly affected by resonance damping than by propagation loss in the substrate. An ErAs:GaAs nanoisland superlattice substrate is shown to allow ultrafast control with a switching recovery time of {approx}10 ps. We also present resonant terahertz transmission in a hybrid plasmonic film comprised of an integrated array of subwavelength metallic islands and semiconductor holes. A large dynamic transition between a dipolar localized surface plasmon mode and a surface plasmon resonance near 0.8 THz is observed under near infrared optical excitation. The reversal in transmission amplitude from a stopband to a passband and up to {pi}/2 phase shift achieved in the hybrid plasmonic film make it promising in large dynamic phase modulation, optical changeover switching, and active terahertz plasmonics.

Analysis of Irradiation Holes of In-Core Region

Energy Technology Data Exchange (ETDEWEB)

In, Won-ho; Lee, Yong-sub; Kim, Tae-hwan; Lim, Kyoung-hwan; Ahn, Hyung-jin [Korea Atomic Energy Research Institute, Daejeon (Korea, Republic of)

2015-05-15

Test fuels and materials are irradiated in the in-core region in side of the chimney. The inner chimney is composed of In-Core and Out-Core regions. The In-Core region has 23 hexagonal vertical irradiation holes named from R01 to R20, CT, IR1 and IR2 and 8 cylindrical irradiation holes named from CAR1 to CAR4 and SOR1 to SOR4. The Out-Core region is composed of 8 cylindrical irradiation holes named from OR1 to OR8 which are installed near the inner shell of the reflector tank. HANARO is the multi-purpose research reactor which utilizes in-core irradiation holes, which is being used in various field. Over the past 7 years we have used CT 8 times, IR once, IR2 and OR3 twice, OR4 three times and OR5 ten times. These irradiation holes are used to perform an evaluation of the neutron irradiation properties and the tests were all completed and done successfully. HANARO has been used successfully, and it still will be used continuously in various fields such as nuclear in-pile tests, the production of radioisotopes, neutron transmutation doping, neutron activation analysis, neutron beam research, radiography, environmental science.

Use of interfacial layers to prolong hole lifetimes in hematite probed by ultrafast transient absorption spectroscopy

Science.gov (United States)

Paradzah, Alexander T.; Diale, Mmantsae; Maabong, Kelebogile; Krüger, Tjaart P. J.

2018-04-01

Hematite is a widely investigated material for applications in solar water oxidation due primarily to its small bandgap. However, full realization of the material continues to be hampered by fast electron-hole recombination rates among other weaknesses such as low hole mobility, short hole diffusion length and low conductivity. To address the problem of fast electron-hole recombination, researchers have resorted to growth of nano-structured hematite, doping and use of under-layers. Under-layer materials enhance the photo-current by minimising electron-hole recombination through suppressing of back electron flow from the substrate, such as fluorine-doped tin oxide (FTO), to hematite. We have carried out ultrafast transient absorption spectroscopy on hematite in which Nb2O5 and SnO2 materials were used as interfacial layers to enhance hole lifetimes. The transient absorption data was fit with four different lifetimes ranging from a few hundred femtoseconds to a few nanoseconds. We show that the electron-hole recombination is slower in samples where interfacial layers are used than in pristine hematite. We also develop a model through target analysis to illustrate the effect of under-layers on electron-hole recombination rates in hematite thin films.

Ultrafast Raman scattering in gas-filled hollow-core fibers

OpenAIRE

Belli, Federico

2017-01-01

The experimental and numerical work reported here is rooted in ultrafast molecular phenomena and nonlinear fiber optics, which are brought together in a deceptively simple system: a homo-nuclear molecular gas (e.g. H2,D2) loaded in the hollow-core of a broad-band guiding photonic crystal fiber (PCF) and exposed to ultrashort pulses of moderate energies (∼ μJ). On one hand, the choice of a molecular gas as the nonlinear medium provides a rich playground for light-matter interactions. ...

Hole-hole correlations in the U=∞ limit of the Hubbard model and the stability of the Nagaoka state

International Nuclear Information System (INIS)

Long, M.W.; Zotos, X.

1993-01-01

We use exact diagonalization in order to study the infinite-U limit of the two-dimensional Hubbard model. As well as looking at single-particle correlations, such as n kσ =left-angle c kσ † c kσ right-angle, we also study N-particle correlation functions, which compare the relative positions of all the particles in different models. In particular we study 16- and 18-site clusters and compare the charge correlations in the Hubbard model with those of spinless fermions and hard-core bosons. We find that although low densities of holes favor a ''locally ferromagnetic'' fermionic description, the correlations at larger densities resemble those of pure hard-core bosons surprisingly well

Soliton-based ultrafast multi-wavelength nonlinear switching in dual-core photonic crystal fibre

International Nuclear Information System (INIS)

Stajanca, P; Pysz, D; Michalka, M; Bugar, I; Andriukaitis, G; Balciunas, T; Fan, G; Baltuska, A

2014-01-01

Systematic experimental study of ultrafast multi-wavelength all-optical switching performance in a dual-core photonic crystal fibre is presented. The focus is on nonlinearly induced switching between the two output ports at non-excitation wavelengths, which are generated during nonlinear propagation of femtosecond pulses in the anomalous dispersion region of a dual-core photonic crystal fibre made of multicomponent glass. Spatial and spectral characteristics of the fibre output radiation were measured separately for both fibre cores under various polarization and intensity conditions upon selective, individual excitation of each fibre core. Polarization-controlled nonlinear switching performance at multiple non-excitation wavelengths was demonstrated in the long-wavelength optical communication bands and beyond. Depending on the input pulse polarization, narrowband switching operation at 1560 nm and 1730 nm takes place with double core extinction ratio contrasts of 9 dB and 14.5 dB, respectively. Moreover, our approach allows switching with simultaneous wavelength shift from 1650 to 1775 nm with extinction ratio contrast larger than 18 dB. In addition, non-reciprocal behaviour of the soliton fission process under different fibre core excitations was observed and its effect on the multi-wavelength nonlinear switching performance was explained, taking into account the slight dual-core structure asymmetry. The obtained results represent ultrafast all-optical switching with an extended dimension of wavelength shift, controllable with both the input radiation intensity and the polarization by simple propagation along a 14 mm long fibre. (paper)

Ultrafast exciton decay in PbS quantum dots through simultaneous electron and hole recombination with a surface-localized ion pair

Energy Technology Data Exchange (ETDEWEB)

Edme, Kedy; Bettis Homan, Stephanie; Nepomnyashchii, Alexander B.; Weiss, Emily A., E-mail: e-weiss@northwestern.edu

2016-06-01

Highlights: • We synthesize complexes of PbS quantum dots (QDs) and tetracyanoquinodimethane (TCNQ). Each PbS QD spontaneously reduces up to 17 TCNQ molecules. • The photoluminescence of the PbS QDs is quenched in the presence of the reduced TCNQ species through ultrafast non-radiative, simultaneous decay of the electron and hole. • We assign this decay to a four-carrier, concerted charge recombination mechanism with the surface localized sulfur–TCNQ{sup x−} ion pair. - Abstract: This paper describes the ultrafast decay of the band-edge exciton in PbS quantum dots (QDs) through simultaneous recombination of the excitonic hole and electron with the surface localized ion pair formed upon adsorption of tetracyanoquinodimethane (TCNQ). Each PbS QD (R = 1.8 nm) spontaneously reduces up to 17 TCNQ molecules upon adsorption of the TCNQ molecule to a sulfur on the QD surface. The photoluminescence of the PbS QDs is quenched in the presence of the reduced TCNQ species through ultrafast (⩽15-ps) non-radiative decay of the exciton; the rate constant for the decay process increases approximately linearly with the number of adsorbed, reduced TCNQ molecules. Near-infrared and mid-infrared transient absorption show that this decay occurs through simultaneous transfer of the excitonic electron and hole, and is assigned to a four-carrier, concerted charge recombination mechanism based on the observations that (i) the PL of the QDs recovers when spontaneously reduced TCNQ{sup 1−} desorbs from the QD surface upon addition of salt, and (ii) the PL of the QDs is preserved when another spontaneous oxidant, ferrocinium, which cannot participate in charge transfer in its reduced state, is substituted for TCNQ.

Disentangling formation of multiple-core holes in aminophenol molecules exposed to bright X-FEL radiation

International Nuclear Information System (INIS)

Zhaunerchyk, V; Squibb, R J; Eland, J H D; Kamińska, M; Mucke, M; Piancastelli, M N; Frasinski, L J; Grilj, J; Koch, M; McFarland, B K; Sistrunk, E; Gühr, M; Coffee, R N; Bostedt, C; Bozek, J D; Salén, P; Meulen, P v d; Linusson, P; Thomas, R D; Larsson, M

2015-01-01

Competing multi-photon ionization processes, some leading to the formation of double core hole states, have been examined in 4-aminophenol. The experiments used the linac coherent light source (LCLS) x-ray free electron laser, in combination with a time-of-flight magnetic bottle electron spectrometer and the correlation analysis method of covariance mapping. The results imply that 4-aminophenol molecules exposed to the focused x-ray pulses of the LCLS sequentially absorb more than two x-ray photons, resulting in the formation of multiple core holes as well as in the sequential removal of photoelectrons and Auger electrons (so-called PAPA sequences). (paper)

Ultrafast dynamics of Coulomb correlated excitons in GaAs quantum wells

Energy Technology Data Exchange (ETDEWEB)

Mycek, M.A. [Univ. of California, Berkeley, CA (United States). Dept. of Physics]|[Lawrence Berkeley National Lab., CA (United States). Materials Sciences Div.

1995-12-01

The author measures the transient nonlinear optical response of room temperature excitons in gallium arsenide quantum wells via multi-wave mixing experiments. The dynamics of the resonantly excited excitons is directly reflected by the ultrafast decay of the induced nonlinear polarization, which radiates the detected multi-wave mixing signal. She characterizes this ultrafast coherent emission in both amplitude and phase, using time- and frequency-domain measurement techniques, to better understand the role of Coulomb correlation in these systems. To interpret the experimental results, the nonlinear optical response of a dense medium is calculated using a model including Coulomb interaction. She contributes three new elements to previous theoretical and experimental studies of these systems. First, surpassing traditional time-integrated measurements, she temporally resolves the amplitude of the ultrafast coherent emission. Second, in addition to measuring the third-order four-wave mixing signal, she also investigates the fifth-order six-wave mixing response. Third, she characterizes the ultrafast phase dynamics of the nonlinear emission using interferometric techniques with an unprecedented resolution of approximately 140 attoseconds. The author finds that effects arising from Coulomb correlation dominate the nonlinear optical response when the density of excitons falls below 3 {times} 10{sup 11} cm{sup {minus}2}, the saturation density. These signatures of Coulomb correlation are investigated for increasing excitation density to gradually screen the interactions and test the validity of the model for dense media. The results are found to be qualitatively consistent with both the predictions of the model and with numerical solutions to the semiconductor Bloch equations. Importantly, the results also indicate current experimental and theoretical limitations, which should be addressed in future research.

Ultrafast Time-Resolved Photoluminescence Studies of Gallium-Arsenide

Science.gov (United States)

Johnson, Matthew Bruce

This thesis concerns the study of ultrafast phenomena in GaAs using time-resolved photoluminescence (PL). The thesis consists of five chapters. Chapter one is an introduction, which discusses the study of ultrafast phenomena in semiconductors. Chapter two is a description of the colliding-pulse mode-locked (CPM) ring dye laser, which is at the heart of the experimental apparatus used in this thesis. Chapter three presents a detailed experimental and theoretical investigation of photoluminescence excitation correlation spectroscopy (PECS), the novel technique which is used to time-resolve ultrafast PL phenomena. Chapters 4 and 5 discuss two applications of the PECS technique. In Chapter 4 the variation of PL intensity in In-alloyed GaAs substrate material is studied, while Chapter 5 discusses the variation of carrier lifetimes in ion-damaged GaAs used in photo-conductive circuit elements (PCEs). PECS is a pulse-probe technique that measures the cross correlation of photo-excited carrier populations. The theoretical model employed in this thesis is based upon the rate equation for a simple three-level system consisting of valence and conduction bands and a single trap level. In the limit of radiative band-to-band dominated recombination, no PECS signal should be observed; while in the capture -dominated recombination limit, the PECS signal from the band-to-band PL measures the cross correlation of the excited electron and hole populations and thus, the electron and hole lifetimes. PECS is experimentally investigated using a case study of PL in semi-insulating (SI) GaAs and In -alloyed GaAs. At 77 K, the PECS signal is characteristic of a capture-dominated system, yielding an electron-hole lifetime of about 200 ps. However, at 5 K the behavior is more complicated and shows saturation effects due to the C acceptor level, which is un-ionized at 5 K. As a first application, PECS is used to investigate the large band-to-band PL contrast observed near dislocations in In

Ultrafast Hierarchical OTDM/WDM Network

Directory of Open Access Journals (Sweden)

Hideyuki Sotobayashi

2003-12-01

Full Text Available Ultrafast hierarchical OTDM/WDM network is proposed for the future core-network. We review its enabling technologies: C- and L-wavelength-band generation, OTDM-WDM mutual multiplexing format conversions, and ultrafast OTDM wavelengthband conversions.

Drilling history of core hole DB-15

International Nuclear Information System (INIS)

Diediker, L.D.; Ledgerwood, R.K.

1980-09-01

This core hole was drilled to obtain hydrologic and chemical data on the permeable zones of the Saddle Mountains and Wanapum Formations. These data were obtained by testing the zones that were penetrated during drilling. This testing-as-drilled method reduced the potential problems of interflow and water contamination. This report summarizes the drilling and coring operations; geologic logging, hydrologic testing, and geophysical logging activities; and cementing operations of DB-15 during drilling. The successful completion of DB-15 demonstrated that hydrologic testing can be conducted during core drilling operations. More reliable head measurements and uncontaminated representative water samples from isolated permeable zones, which have not been exposed to potential open borehole cross-flow and head equilibration problems, were benefits derived from the testing-as-drilled method. Disadvantages of the technique were a longer time to complete the borehole caused by time required for testing and increased drilling costs due to rig standby time during testing. Extension of the testing-as-drilled method to the drilling of future core holes is recommended. An evaluation should be made of the required hydrologic data and expected borehole stratigraphy before and during drilling to allow uninterrupted drilling in zones of low permeability that can be tested after drilling is complete

Nonlinear performance of asymmetric coupler based on dual-core photonic crystal fiber: Towards sub-nanojoule solitonic ultrafast all-optical switching

Science.gov (United States)

Curilla, L.; Astrauskas, I.; Pugzlys, A.; Stajanca, P.; Pysz, D.; Uherek, F.; Baltuska, A.; Bugar, I.

2018-05-01

We demonstrate ultrafast soliton-based nonlinear balancing of dual-core asymmetry in highly nonlinear photonic crystal fiber at sub-nanojoule pulse energy level. The effect of fiber asymmetry was studied experimentally by selective excitation and monitoring of individual fiber cores at different wavelengths between 1500 nm and 1800 nm. Higher energy transfer rate to non-excited core was observed in the case of fast core excitation due to nonlinear asymmetry balancing of temporal solitons, which was confirmed by the dedicated numerical simulations based on the coupled generalized nonlinear Schrödinger equations. Moreover, the simulation results correspond qualitatively with the experimentally acquired dependences of the output dual-core extinction ratio on excitation energy and wavelength. In the case of 1800 nm fast core excitation, narrow band spectral intensity switching between the output channels was registered with contrast of 23 dB. The switching was achieved by the change of the excitation pulse energy in sub-nanojoule region. The performed detailed analysis of the nonlinear balancing of dual-core asymmetry in solitonic propagation regime opens new perspectives for the development of ultrafast nonlinear all-optical switching devices.

Interpretation of photocurrent correlation measurements used for ultrafast photoconductive switch characterization

DEFF Research Database (Denmark)

Jacobsen, R. H.; Birkelund, Karen; Holst, T.

1996-01-01

of the switch. By using both photocurrent measurements and terahertz spectroscopy we verify the importance of space-charge effects on the carrier dynamics. Photocurrent nonlinearities and coherent effects are discussed as they appear in the correlation signals. An analysis based on a simple model allows......Photocurrent correlation measurements used for the characterization of ultrafast photoconductive switches based on GaAs and silicon-on-sapphire are demonstrated. The correlation signal arises from the interplay of the photoexcited carriers, the dynamics of the bias field and a subsequent recharging...

Ultrafast Spectroscopy of Semiconductor Devices

DEFF Research Database (Denmark)

Borri, Paola; Langbein, Wolfgang; Hvam, Jørn Marcher

1999-01-01

In this work we present an experimental technique for investigating ultrafast carrier dynamics in semiconductor optical amplifiers at room temperature. These dynamics, influenced by carrier heating, spectral hole-burning and two-photon absorption, are very important for device applications in inf...

X-ray atomic scattering factors of low-Z ions with a core hole

International Nuclear Information System (INIS)

Hau-Riege, Stefan P.

2007-01-01

Short and intense x-ray pulses may be used for atomic-resolution diffraction imaging of single biological molecules. One of the dominant damage mechanisms is atomic ionization, resulting in a large fraction of atoms with core holes. We calculated the atomic scattering factor of atoms with atomic charge numbers between 3 and 10 in different ionization states with and without a core hole. Our results show that orbital occupation and the change of the orbitals upon core ionization (core relaxation) have a significant impact on the diffraction pattern

Xclaim: A graphical interface for the calculation of core-hole spectroscopies

International Nuclear Information System (INIS)

Fernández-Rodríguez, Javier; Toby, Brian; Veenendaal, Michel van

2015-01-01

Highlights: • The program Xclaim (X-ray core level atomic multiplets) calculates core-hole spectra. • Crystal field under an arbitrary point symmetry and hybridization with ligands. • X-ray absorption spectroscopy (XAS), X-ray photoemission spectroscopy (XPS), photoemission spectroscopy (PES) and inverse photoemission (IPES). - Abstract: Xclaim (X-ray core level atomic multiplets) is a graphical interface for the calculation of core-hole spectroscopy and ground state properties within a charge-transfer multiplet model taking into account a many-body Hamiltonian with Coulomb, spin–orbit, crystal-field, and hybridization interactions. Using Coulomb and spin–orbit parameters calculated in the Hartree–Fock limit and ligand field parameters (crystal-field, hybridization and charge-transfer energy) the program calculates X-ray absorption spectroscopy (XAS), X-ray photoemission spectroscopy (XPS), photoemission spectroscopy (PES) and inverse photoemission (IPES). The program runs on Linux, Windows and MacOS platforms

Xclaim: A graphical interface for the calculation of core-hole spectroscopies

Energy Technology Data Exchange (ETDEWEB)

Fernández-Rodríguez, Javier [Department of Physics, Northern Illinois University, DeKalb, IL 60115 (United States); Advanced Photon Source, Argonne National Laboratory, 9700 South Cass Avenue, Argonne, IL 60439 (United States); Toby, Brian, E-mail: toby@anl.gov [Advanced Photon Source, Argonne National Laboratory, 9700 South Cass Avenue, Argonne, IL 60439 (United States); Veenendaal, Michel van, E-mail: veenendaal@niu.edu [Department of Physics, Northern Illinois University, DeKalb, IL 60115 (United States); Advanced Photon Source, Argonne National Laboratory, 9700 South Cass Avenue, Argonne, IL 60439 (United States)

2015-07-15

Highlights: • The program Xclaim (X-ray core level atomic multiplets) calculates core-hole spectra. • Crystal field under an arbitrary point symmetry and hybridization with ligands. • X-ray absorption spectroscopy (XAS), X-ray photoemission spectroscopy (XPS), photoemission spectroscopy (PES) and inverse photoemission (IPES). - Abstract: Xclaim (X-ray core level atomic multiplets) is a graphical interface for the calculation of core-hole spectroscopy and ground state properties within a charge-transfer multiplet model taking into account a many-body Hamiltonian with Coulomb, spin–orbit, crystal-field, and hybridization interactions. Using Coulomb and spin–orbit parameters calculated in the Hartree–Fock limit and ligand field parameters (crystal-field, hybridization and charge-transfer energy) the program calculates X-ray absorption spectroscopy (XAS), X-ray photoemission spectroscopy (XPS), photoemission spectroscopy (PES) and inverse photoemission (IPES). The program runs on Linux, Windows and MacOS platforms.

Influence of heat treatment on hole transfer dynamics in core-shell quantum dot/organic hole conductor hybrid films

Science.gov (United States)

Sun, Mingye; Zheng, Youjin; Zhang, Lei; Zhao, Liping; Zhang, Bing

2017-08-01

The influence of heat treatment on hole transfer (HT) processes from the CdSe/ZnS and CdSe/CdS/ZnS quantum dots (QDs) to 4,4‧,4″-Tris(carbazol-9-yl)-triphenylamine (TCTA) in QD/TCTA hybrid films has been researched with time-resolved photoluminescence (PL) spectroscopy. The PL dynamic results demonstrated a heat-treatment-temperature-dependent HT process from the core-shell CdSe QDs to TCTA. The HT rates and efficiencies can be effectively increased due to reduced distance between core-shell CdSe QDs and TCTA after heat treatment. The CdS shell exhibited a more obvious effect on HT from the core-shell CdSe QDs to TCTA than on electron transfer to TiO2, due to higher barrier for holes to tunnel through CdS shell and larger effective mass of holes in CdS than electrons. These results indicate that heat treatment would be an effective means to further optimize solid-state QD sensitized solar cells and rational design of CdS shell is significant.

Selecting core-hole localization or delocalization in CS2 by photofragmentation dynamics.

Science.gov (United States)

Guillemin, R; Decleva, P; Stener, M; Bomme, C; Marin, T; Journel, L; Marchenko, T; Kushawaha, R K; Jänkälä, K; Trcera, N; Bowen, K P; Lindle, D W; Piancastelli, M N; Simon, M

2015-01-21

Electronic core levels in molecules are highly localized around one atomic site. However, in single-photon ionization of symmetric molecules, the question of core-hole localization versus delocalization over two equivalent atoms has long been debated as the answer lies at the heart of quantum mechanics. Here, using a joint experimental and theoretical study of core-ionized carbon disulfide (CS2), we demonstrate that it is possible to experimentally select distinct molecular-fragmentation pathways in which the core hole can be considered as either localized on one sulfur atom or delocalized between two indistinguishable sulfur atoms. This feat is accomplished by measuring photoelectron angular distributions within the frame of the molecule, directly probing entanglement or disentanglement of quantum pathways as a function of how the molecule dissociates.

Ultrafast Holographic Image Recording by Single Shot Femtosecond Spectral Hole Burning

National Research Council Canada - National Science Library

Rebane, Aleksander

2001-01-01

.... This allowed us to record image holograms with 150-fs duration pulses without need to accumulate the SHB effect from many exposures. Results of this research show that it is possible to perform optical recording of data in frequency-domain on ultrafast time scale. These results can be used also as a new diagnostic tool for femtosecond dynamics in various ultrafast optical interactions.

Observation of hole accumulation in Ge/Si core/shell nanowires using off-axis electron holography.

Science.gov (United States)

Li, Luying; Smith, David J; Dailey, Eric; Madras, Prashanth; Drucker, Jeff; McCartney, Martha R

2011-02-09

Hole accumulation in Ge/Si core/shell nanowires (NWs) has been observed and quantified using off-axis electron holography and other electron microscopy techniques. The epitaxial [110]-oriented Ge/Si core/shell NWs were grown on Si (111) substrates by chemical vapor deposition through the vapor-liquid-solid growth mechanism. High-angle annular-dark-field scanning transmission electron microscopy images and off-axis electron holograms were obtained from specific NWs. The excess phase shifts measured by electron holography across the NWs indicated the presence of holes inside the Ge cores. Calculations based on a simplified coaxial cylindrical model gave hole densities of (0.4 ± 0.2) /nm(3) in the core regions.

Supermassive black holes do not correlate with galaxy disks or pseudobulges.

Science.gov (United States)

Kormendy, John; Bender, R; Cornell, M E

2011-01-20

The masses of supermassive black holes are known to correlate with the properties of the bulge components of their host galaxies. In contrast, they seem not to correlate with galaxy disks. Disk-grown 'pseudobulges' are intermediate in properties between bulges and disks; it has been unclear whether they do or do not correlate with black holes in the same way that bulges do. At stake in this issue are conclusions about which parts of galaxies coevolve with black holes, possibly by being regulated by energy feedback from black holes. Here we report pseudobulge classifications for galaxies with dynamically detected black holes and combine them with recent measurements of velocity dispersions in the biggest bulgeless galaxies. These data confirm that black holes do not correlate with disks and show that they correlate little or not at all with pseudobulges. We suggest that there are two different modes of black-hole feeding. Black holes in bulges grow rapidly to high masses when mergers drive gas infall that feeds quasar-like events. In contrast, small black holes in bulgeless galaxies and in galaxies with pseudobulges grow as low-level Seyfert galaxies. Growth of the former is driven by global processes, so the biggest black holes coevolve with bulges, but growth of the latter is driven locally and stochastically, and they do not coevolve with disks and pseudobulges.

Atomistic Tight-Binding Theory of Electron-Hole Exchange Interaction in Morphological Evolution of CdSe/ZnS Core/Shell Nanodisk to CdSe/ZnS Core/Shell Nanorod

Directory of Open Access Journals (Sweden)

Worasak Sukkabot

2016-01-01

Full Text Available Based on the atomistic tight-binding theory (TB and a configuration interaction (CI description, the electron-hole exchange interaction in the morphological transformation of CdSe/ZnS core/shell nanodisk to CdSe/ZnS core/shell nanorod is described with the aim of understanding the impact of the structural shapes on the change of the electron-hole exchange interaction. Normally, the ground hole states confined in typical CdSe/ZnS core/shell nanocrystals are of heavy hole-like character. However, the atomistic tight-binding theory shows that a transition of the ground hole states from heavy hole-like to light hole-like contribution with the increasing aspect ratios of the CdSe/ZnS core/shell nanostructures is recognized. According to the change in the ground-state hole characters, the electron-hole exchange interaction is also significantly altered. To do so, optical band gaps, ground-state electron character, ground-state hole character, oscillation strengths, ground-state coulomb energies, ground-state exchange energies, and dark-bright (DB excitonic splitting (stoke shift are numerically demonstrated. These atomistic computations obviously show the sensitivity with the aspect ratios. Finally, the alteration in the hole character has a prominent effect on dark-bright (DB excitonic splitting.

Ultrafast Control of Magnetism in Ferromagnetic Semiconductors via Photoexcited Transient Carriers

Energy Technology Data Exchange (ETDEWEB)

Cotoros, Ingrid A. [Univ. of California, Berkeley, CA (United States)

2008-12-01

The field of spintronics offers perspectives for seamless integration of coupled and inter-tunable electrical and magnetic properties in a single device. For integration of the spin degree of freedom with current electronic technology, new semiconductors are needed that show electrically-tunable magnetic properties at room temperature and above. Dilute magnetic semiconductors derived from III-V compounds, like GaMnAs and InMnAs, show coupled and tunable magnetic, transport, and optical properties, due to the fact that their ferromagnetism is hole-mediated. These unconventional materials are ideal systems for manipulating the magnetic order by changing the carrier polarization, population density, and energy band distribution of the complementary subsystem of holes. This is the main theme we cover in this thesis. In particular, we develop a unique setup by use of ultraviolet pump, near-infrared probe femtosecond laser pulses, that allows for magneto-optical Kerr effect (MOKE) spectroscopy experiments. We photo-excite transient carriers in our samples, and measure the induced transient magnetization dynamics. One set of experiments performed allowed us to observe for the first time enhancement of the ferromagnetic order in GaMnAs, on an ultrafast time scale of hundreds of picoseconds. The corresponding transient increase of Curie temperature (Tc, the temperature above which a ferromagnetic material loses its permanent magnetism) of about 1 K for our experimental conditions is a very promising result for potential spintronics applications, especially since it is seconded by observation of an ultrafast ferromagnetic to paramagnetic phase transition above Tc. In a different set of experiments, we "write" the magnetization in a particular orientation in the sample plane. Using an ultrafast scheme, we alter the distribution of holes in the system and detect signatures of the particular memory state in the subsequent magnetization dynamics, with unprecedented hundreds of

Supermassive black holes do not correlate with dark matter haloes of galaxies.

Science.gov (United States)

Kormendy, John; Bender, Ralf

2011-01-20

Supermassive black holes have been detected in all galaxies that contain bulge components when the galaxies observed were close enough that the searches were feasible. Together with the observation that bigger black holes live in bigger bulges, this has led to the belief that black-hole growth and bulge formation regulate each other. That is, black holes and bulges coevolve. Therefore, reports of a similar correlation between black holes and the dark matter haloes in which visible galaxies are embedded have profound implications. Dark matter is likely to be non-baryonic, so these reports suggest that unknown, exotic physics controls black-hole growth. Here we show, in part on the basis of recent measurements of bulgeless galaxies, that there is almost no correlation between dark matter and parameters that measure black holes unless the galaxy also contains a bulge. We conclude that black holes do not correlate directly with dark matter. They do not correlate with galaxy disks, either. Therefore, black holes coevolve only with bulges. This simplifies the puzzle of their coevolution by focusing attention on purely baryonic processes in the galaxy mergers that make bulges.

Supplemental materials for the ICDP-USGS Eyreville A, B, and C core holes, Chesapeake Bay impact structure: Core-box photographs, coring-run tables, and depth-conversion files

Science.gov (United States)

Durand, C.T.; Edwards, L.E.; Malinconico, M.L.; Powars, D.S.

2009-01-01

During 2005-2006, the International Continental Scientific Drilling Program and the U.S. Geological Survey drilled three continuous core holes into the Chesapeake Bay impact structure to a total depth of 1766.3 m. A collection of supplemental materials that presents a record of the core recovery and measurement data for the Eyreville cores is available on CD-ROM at the end of this volume and in the GSA Data Repository. The supplemental materials on the CD-ROM include digital photographs of each core box from the three core holes, tables of the three coring-run logs, as recorded on site, and a set of depth-conversion programs. In this chapter, the contents, purposes, and basic applications of the supplemental materials are briefly described. With this information, users can quickly decide if the materials will apply to their specific research needs. ?? 2009 The Geological Society of America.

Cascading electron and hole transfer dynamics in a CdS/CdTe core-shell sensitized with bromo-pyrogallol red (Br-PGR): slow charge recombination in type II regime.

Science.gov (United States)

Maity, Partha; Debnath, Tushar; Chopra, Uday; Ghosh, Hirendra Nath

2015-02-14

Ultrafast cascading hole and electron transfer dynamics have been demonstrated in a CdS/CdTe type II core-shell sensitized with Br-PGR using transient absorption spectroscopy and the charge recombination dynamics have been compared with those of CdS/Br-PGR composite materials. Steady state optical absorption studies suggest that Br-PGR forms strong charge transfer (CT) complexes with both the CdS QD and CdS/CdTe core-shell. Hole transfer from the photo-excited QD and QD core-shell to Br-PGR was confirmed by both steady state and time-resolved emission spectroscopy. Charge separation was also confirmed by detecting electrons in the conduction band of the QD and the cation radical of Br-PGR as measured from femtosecond transient absorption spectroscopy. Charge separation in the CdS/Br-PGR composite materials was found to take place in three different pathways, by transferring the photo-excited hole of CdS to Br-PGR, electron injection from the photo-excited Br-PGR to the CdS QD, and direct electron transfer from the HOMO of Br-PGR to the conduction band of the CdS QD. However, in the CdS/CdTe/Br-PGR system hole transfer from the photo-excited CdS to Br-PGR and electron injection from the photo-excited Br-PGR to CdS take place after cascading through the CdTe shell QD. Charge separation also takes place via direct electron transfer from the Br-PGR HOMO to the conduction band of CdS/CdTe. Charge recombination (CR) dynamics between the electron in the conduction band of the CdS QD and the Br-PGR cation radical were determined by monitoring the bleach recovery kinetics. The CR dynamics were found to be much slower in the CdS/CdTe/Br-PGR system than in the CdS/Br-PGR system. The formation of the strong CT complex and the separation of charges cascading through the CdTe shell help to slow down charge recombination in the type II regime.

Ultrafast photoinduced charge separation in metal-semiconductor nanohybrids.

Science.gov (United States)

Mongin, Denis; Shaviv, Ehud; Maioli, Paolo; Crut, Aurélien; Banin, Uri; Del Fatti, Natalia; Vallée, Fabrice

2012-08-28

Hybrid nano-objects formed by two or more disparate materials are among the most promising and versatile nanosystems. A key parameter in their properties is interaction between their components. In this context we have investigated ultrafast charge separation in semiconductor-metal nanohybrids using a model system of gold-tipped CdS nanorods in a matchstick architecture. Experiments are performed using an optical time-resolved pump-probe technique, exciting either the semiconductor or the metal component of the particles, and probing the light-induced change of their optical response. Electron-hole pairs photoexcited in the semiconductor part of the nanohybrids are shown to undergo rapid charge separation with the electron transferred to the metal part on a sub-20 fs time scale. This ultrafast gold charging leads to a transient red-shift and broadening of the metal surface plasmon resonance, in agreement with results for free clusters but in contrast to observation for static charging of gold nanoparticles in liquid environments. Quantitative comparison with a theoretical model is in excellent agreement with the experimental results, confirming photoexcitation of one electron-hole pair per nanohybrid followed by ultrafast charge separation. The results also point to the utilization of such metal-semiconductor nanohybrids in light-harvesting applications and in photocatalysis.

Lifetime broadening of atomic lines produced upon ultrafast dissociation of HCl and HBr

Energy Technology Data Exchange (ETDEWEB)

Lablanquie, P., E-mail: pascal.lablanquie@upmc.fr [Sorbonne Universités, UPMC Univ Paris 06, LCPMR, 11 rue Pierre et Marie Curie, 75231 Paris Cedex 05 (France); CNRS, LCPMR (UMR 7614), 11 rue Pierre et Marie Curie, 75231 Paris Cedex 05 (France); Iwayama, H. [UVSOR Facility, Institute for Molecular Science, Okazaki 444-8585 (Japan); Penent, F. [Sorbonne Universités, UPMC Univ Paris 06, LCPMR, 11 rue Pierre et Marie Curie, 75231 Paris Cedex 05 (France); CNRS, LCPMR (UMR 7614), 11 rue Pierre et Marie Curie, 75231 Paris Cedex 05 (France); Soejima, K. [Department of Environmental Science, Niigata University, Niigata 950-2181 (Japan); Shigemasa, E. [UVSOR Facility, Institute for Molecular Science, Okazaki 444-8585 (Japan)

2014-08-15

Highlights: • Ultrafast dissociation of HCl is triggered by 2p{sub 3/2} → σ* excitation. • Ultrafast dissociation of HBr is triggered by 3d{sub 5/2} → σ* excitation. • Photoelectron spectroscopy reveals sharp vibrational molecular lines and broad atomic lines. • The profiles of the atomic lines are analyzed in detail. • We extract the lifetime of the inner shell hole in the neutral atomic fragment. - Abstract: Ultrafast dissociation of the HCl and HBr molecules excited respectively to the 2p{sub 3/2} → σ* and 3d{sub 5/2} → σ* resonances are studied with high resolution photoelectron spectroscopy. Sharp vibrational molecular lines and broad atomic lines are observed. The analysis of the profile of the atomic lines gives access to the lifetimes of the inner shell 2p{sub 3/2} hole in the Cl* (2p{sub 3/2}){sup −1} 3s{sup 2}3p{sup 6} configuration, and the inner shell 3d{sub 5/2} hole in the Br* (3d{sub 5/2}){sup −1} 4s{sup 2}4p{sup 6} configuration.

Geologic description of cores from holes P-3 MH-1 through P-3 MH-5, Area G, Technical Area 54

International Nuclear Information System (INIS)

Purtymun, W.D.; Wheeler, M.L.; Rogers, M.A.

1978-05-01

Five horizontal holes were cored beneath Pit 3 near the southeast edge of Mesita del Buey at Area G. The pit, filled and covered by 1966, contains solid radioactive wastes. The holes were cored to obtain samples of the tuff underlying the pit to determine if there has been any migration of radionuclides by infiltration of water in the past 10 y. The five holes were collared in Unit 2b of the Tshirege Member of the Bandelier Tuff; three of the holes plunged downward into Unit 2a. This report describes the rock units penetrated by core holes and the joint characteristics observed. The locations of core samples selected for analyses are related to the floor of the pit

EFFECT OF PILOT HOLE TAPPING ON PULLOUT STRENGTH AND INSERTION TORQUE OF DUAL CORE PEDICLE SCREWS.

Science.gov (United States)

Rosa, Rodrigo César; Silva, Patrícia; Falcai, Maurício José; Shimano, Antônio Carlos; Defino, Helton Luiz Aparecido

2010-01-01

To evaluate the influence of pilot hole tapping on pullout resistance and insertion torque of pedicle screws with a conical core. Mechanical tests using a universal testing machine were performed on pedicle screws with a conical core that were inserted into pedicles in the fifth lumbar vertebra of calves. The insertion torque was measured using a torque meter with a capacity of 10 Nm, which was considered to be the highest torque value. The pilot holes were prepared using a probe of external diameter 3.8 mm and tapping of the same dimensions and thread characteristics as the screw. Decreased insertion torque and pullout resistance were observed in the group with prior tapping of the pilot hole. Pilot hole tapping reduced the insertion torque and pullout resistance of pedicle screws with a conical core that had been inserted into the pedicle of the fifth lumbar vertebra of calves.

Neutron activation for logging the distribution of gold in bore-hole cores

International Nuclear Information System (INIS)

Rahmanian, H.; Watterson, J.I.W.

1992-01-01

A new method for the non-destructive determination of gold in bore-hole cores has been developed using instrumental neutron activation analysis with a 252 Cf source. The procedure obtains the distribution and concentration of gold along the longitudinal axis of the core i.e. a log of the gold concentration. The accuracy of the method is comparable to fire assay at a level of 2 ppm and has a detection limit of 1 ppm under the conditions used. The assay of the gold is carried out by employing a novel variation of the conventional comparator method using gold wires as both standard and flux monitor. A method is described for logging gold in bore-hole cores using neutron activation with a 160 μg 252 Cf neutron source. The method has a limit of detection of about 1 ppm under the described conditions. (author)

Coulomb drag in electron-hole bilayer: Mass-asymmetry and exchange correlation effects

Science.gov (United States)

Arora, Priya; Singh, Gurvinder; Moudgil, R. K.

2018-04-01

Motivated by a recent experiment by Zheng et al. [App. Phys. Lett. 108, 062102 (2016)] on coulomb drag in electron-hole and hole-hole bilayers based on GaAs/AlGaAs semiconductor heterostructure, we investigate theoretically the influence of mass-asymmetry and temperature-dependence of correlations on the drag rate. The correlation effects are dealt with using the Vignale-Singwi effective inter-layer interaction model which includes correlations through local-field corrections to the bare coulomb interactions. However, in this work, we have incorporated only the intra-layer correlations using the temperature-dependent Hubbard approximation. Our results display a reasonably good agreement with the experimental data. However, it is crucial to include both the electron-hole mass-asymmetry and temperature-dependence of correlations. Mass-asymmetry and correlations are found to result in a substantial enhancement of drag resistivity.

Ultrafast Mid-Infrared Intra-Excitonic Response of Individualized Single-Walled Carbon Nanotubes

International Nuclear Information System (INIS)

Wang, Jigang; Graham, Matt W.; Ma, Yingzhong; Fleming, Graham R.; Kaindl, Robert A.

2009-01-01

The quasi-1D confinement and reduced screening of photoexcited charges in single-walled carbon nanotubes (SWNTs) entails strongly-enhanced Coulomb interactions and exciton binding energies. Such amplified electron-hole (e-h) correlations have important implications for both fundamental physics and optoelectronic applications of nanotubes. The availability of 'individualized' SWNT ensembles with bright and structured luminescence has rendered specific tube chiralities experimentally accessible. In these samples, evidence for excitonic behavior was found in absorption-luminescence maps, two-photon excited luminescence, or ultrafast carrier dynamics. Here, we report ultrafast mid-infrared (mid-IR) studies of individualized SWNTs, evidencing strong photoinduced absorption around 200 meV in semiconducting tubes of (6,5) and (7,5) chiralities. This manifests the observation of quasi-1D intra-excitonic transitions between different relative-momentum states, in agreement with the binding energy and calculated oscillator strength. Our measurements further reveal a saturation of the photoinduced absorption with increasing phase-space filling of the correlated e-h pairs. The transient mid-IR response represents a new tool, unhindered by restrictions of momentum or interband dipole moment, to investigate the density and dynamics of SWNT excitons.

Correlation between choroidal thickness and macular hole

Directory of Open Access Journals (Sweden)

Li-Li Wang

2018-01-01

Full Text Available AIM:To explore the correlation between choroidal thickness and macular hole, and to provide a theoretical basis for diagnosis and treatment of macular hole. METHODS: This study included 40 cases of monocular idiopathic macular hole patients who were treated in ophthalmology of our hospital from June 2015 to June 2016 and 40 cases of healthy people. Sicked eyes of idiopathic macular hole patients(40 eyeswere set as the Group A, uninjured side eyes(40 eyeswere set as the Group B, eyes of 40 cases of healthy people(40 normal eyeswere set as the Group C. Choroidal thickness of macular fovea, macular fovea 1mm, 3mm at 9 points, 4 directions in the upper, lower, nasal and temporal regions were measured through coherent optical tomography of enhanced deep imaging(enhanced depth image optical coherence tomography, EDI-OCT. They were recorded as SFCT, SCT1mm, SCT3mm, ICT1mm, ICT3mm, NCT1mm, NCT3mm, TCT1mm, TCT3mm, and correlation analysis between SFCT and age was analyzed. RESULTS: Average SFCT of Group A, B had no significant difference, data of the Group C was significantly higher than those of the Group A, B, there was statistical significance(P1mm, SCT3mm, ICT1mm, ICT3mm, NCT1mm, NCT3mm, TCT1mm, TCT3mm of the Group A, B had no significant difference(P>0.05, and choroidal thickness at each point of the Group C was significantly higher than that of Group A and B, there was statistical significance(Pr=-0.065, P=0.148; r=-0.057, P=0.658, SFCT of the Group C was negatively correlated with age(r=-0.343, P=0.041. CONCLUSION: The pathogenesis of idiopathic macular hole may be related to the sharp decrease of choroidal thickness, choroidal thickness of uninjured side eyes reduces more sharply than normal population and choroidal vascular metabolism reduces may be pathogenic.

Quantum correlator outside a Schwarzschild black hole

Directory of Open Access Journals (Sweden)

Claudia Buss

2018-01-01

Full Text Available We calculate the quantum correlator in Schwarzschild black hole space–time. We perform the calculation for a scalar field in three different quantum states: Boulware, Unruh and Hartle–Hawking, and for points along a timelike circular geodesic. The results show that the correlator presents a global fourfold singularity structure, which is state-independent. Our results also show the different correlations in the three different quantum states arising in-between the singularities.

Fran Ridge horizontal coring summary report hole UE-25h No. 1, Yucca Mountain Area, Nye County, Nevada

International Nuclear Information System (INIS)

Norris, A.E.; Byers, F.M. Jr.; Merson, T.J.

1986-10-01

Hole UE-25h No. 1 was core drilled during December 1982 and January 1983 within several degrees of due west, 400 ft horizontally into the southeast slope of Fran Ridge at an altitude of 3409 ft. The purpose of the hole was to obtain data pertinent for radionuclide transport studies in the Topopah Spring Member of the Paintbrush Tuff. This unit had been selected previously as the host rock for the potential underground nuclear waste repository at Yucca Mountain, adjacent to the southwestern part of the Nevada Test Site. The hole was core drilled first with air, then with air mist, and finally with air, soap, and water. Many problems were encountered, including sloughing of tuff into the uncased hole, vibration of the drill rods, high rates of bit wear, and lost circulation of drilling fluids. On the basis of experience gained in drilling this hole, ways to improve horizontal coring with air are suggested in this report. All of the recovered core, except those pieces that were wrapped and waxed, were examined for lithophysal content, for fractures, and for fracture-fill mineralization. The results of this examination are given in this report. Core recovery greater than 80% at between 209 and 388 ft permitted a fracture frequency analysis. The results are similar to the fracture frequencies observed in densely welded nonlithophysal tuff from holes USW GU-3 and USW G-4. The fractures in core from UE-25h No. 1 were found to be smooth and nonmineralized or coated with calcite, silica, or manganese oxide. Open fractures with caliche (porous, nonsparry calcite) were not observed beyond 83.5 ft, which corresponds to an overburden depth of 30 ft

Effect of the final-state interaction on the initial core-hole lifetime: the case of the 4s-hole lifetime of Sn metal

International Nuclear Information System (INIS)

Ohno, Masahide

2003-01-01

The first theoretical study of the effect of the final-state interaction on the initial core-hole lifetime is presented. The 4s-hole lifetime width of Sn metal is calculated by an ab-initio atomic many-body theory (Green's function method). When the final-state interaction in the 4p4d two-hole state, created by the 4s -1 -4p -1 4d -1 εf super Coster-Kronig (CK) transition of the initial 4s hole, is explicitly taken into account, the ab-initio atomic many-body calculation of the 4s-hole X-ray photoelectron spectroscopy (XPS) spectrum of Sn atom can provide excellent agreement with experiment in both the 4s-hole energy and the 4s-hole lifetime width. Otherwise, the many-body calculation underestimates considerably the 4s-hole lifetime width. The 4p4d two-hole state interacts strongly with the 4d triple-hole state by the 4p -1 4d -1 -4d -3 εf super CK transition. The interaction affects greatly the initial 4s-hole lifetime width

Composition of rock core from hole AEC-8, New Mexico

International Nuclear Information System (INIS)

Rhoderick, J.E.; Buck, A.D.

1981-12-01

AEC-8 is a borehole about 5000 ft deep located within the Waste Isolation Pilot Plant (WIPP) site in southeastern New Mexico. About 28 ft of rock core from seven depth intervals in this hole was characterized by petrographic examination. This included logging, examination of the rock with a stereomicroscope, examination of thin sections with a polarizing microscope, and examination of each sample by x-ray diffraction

On the ultrafast charge migration and subsequent charge directed reactivity in Cl⋯N halogen-bonded clusters following vertical ionization

International Nuclear Information System (INIS)

Chandra, Sankhabrata; Bhattacharya, Atanu; Periyasamy, Ganga

2015-01-01

In this article, we have presented ultrafast charge transfer dynamics through halogen bonds following vertical ionization of representative halogen bonded clusters. Subsequent hole directed reactivity of the radical cations of halogen bonded clusters is also discussed. Furthermore, we have examined effect of the halogen bond strength on the electron-electron correlation- and relaxation-driven charge migration in halogen bonded complexes. For this study, we have selected A-Cl (A represents F, OH, CN, NH 2 , CF 3 , and COOH substituents) molecules paired with NH 3 (referred as ACl:NH 3 complex): these complexes exhibit halogen bonds. To the best of our knowledge, this is the first report on purely electron correlation- and relaxation-driven ultrafast (attosecond) charge migration dynamics through halogen bonds. Both density functional theory and complete active space self-consistent field theory with 6-31 + G(d, p) basis set are employed for this work. Upon vertical ionization of NCCl⋯NH 3 complex, the hole is predicted to migrate from the NH 3 -end to the ClCN-end of the NCCl⋯NH 3 complex in approximately 0.5 fs on the D 0 cationic surface. This hole migration leads to structural rearrangement of the halogen bonded complex, yielding hydrogen bonding interaction stronger than the halogen bonding interaction on the same cationic surface. Other halogen bonded complexes, such as H 2 NCl:NH 3 , F 3 CCl:NH 3 , and HOOCCl:NH 3 , exhibit similar charge migration following vertical ionization. On the contrary, FCl:NH 3 and HOCl:NH 3 complexes do not exhibit any charge migration following vertical ionization to the D 0 cation state, pointing to interesting halogen bond strength-dependent charge migration

Ultrafast signal processing in quantum dot amplifiers through effective spectral holeburning

DEFF Research Database (Denmark)

Berg, Tommy Winther; Mørk, Jesper; Uskov, A. V.

2002-01-01

suitable for ultrafast signal processing. The basis of this property is that the process of spectral hole burning (SHB) can become very effective. We consider a traveling wave optical amplifier consisting of the dot states, which interact with the optical signal (no inhomogeneous broadening included...

X-ray Fluorescence Core Scanning of Oman Drilling Project Holes BT1B and GT3A Cores on D/V CHIKYU

Science.gov (United States)

Johnson, K. T. M.; Kelemen, P. B.; Michibayashi, K.; Greenberger, R. N.; Koepke, J.; Beinlich, A.; Morishita, T.; Jesus, A. P. M.; Lefay, R.

2017-12-01

The JEOL JSX-3600CA1 energy dispersive X-ray fluorescence core logger (XRF-CL) on the D/V Chikyu provides quantitative element concentrations of scanned cores. Scans of selected intervals are made on an x-y grid with point spacing of 5 mm. Element concentrations for Si, Al, Ti, Ca, Mg, Mn, Fe, Na, K, Cr, Ni, S and Zn are collected for each point on the grid. Accuracy of element concentrations provided by the instrument software is improved by applying empirical correction algorithms. Element concentrations were collected for 9,289 points from twenty-seven core intervals in Hole BT1B (basal thrust) and for 6,389 points from forty core intervals in Hole GT3A (sheeted dike-gabbro transition) of the Oman Drilling Project on the D/V Chikyu XRF-CL during Leg 2 of the Oman Drilling Project in August-September, 2017. The geochemical data are used for evaluating downhole compositional details associated with lithological changes, unit contacts and mineralogical variations and are particularly informative when plotted as concentration contour maps or downhole concentration diagrams. On Leg 2 additional core scans were made with X-ray Computed Tomography (X-ray CT) and infrared images from the visible-shortwave infrared imaging spectroscopy (IR) systems on board. XRF-CL, X-ray CT and IR imaging plots used together provide detailed information on rock compositions, textures and mineralogy that assist naked eye visual observations. Examples of some uses of XRF-CL geochemical maps and downhole data are shown. XRF-CL and IR scans of listvenite clearly show zones of magnesite, dolomite and the Cr-rich mica, fuchsite that are subdued in visual observation, and these scans can be used to calculate variations in proportions of these minerals in Hole BT1B cores. In Hole GT3A XRF-CL data can be used to distinguish compositional changes in different generations of sheeted dikes and gabbros and when combined with visual observations of intrusive relationships the detailed geochemical

Correlation induced electron-hole asymmetry in quasi- two-dimensional iridates.

Science.gov (United States)

Pärschke, Ekaterina M; Wohlfeld, Krzysztof; Foyevtsova, Kateryna; van den Brink, Jeroen

2017-09-25

The resemblance of crystallographic and magnetic structures of the quasi-two-dimensional iridates Ba 2 IrO 4 and Sr 2 IrO 4 to La 2 CuO 4 points at an analogy to cuprate high-Tc superconductors, even if spin-orbit coupling is very strong in iridates. Here we examine this analogy for the motion of a charge (hole or electron) added to the antiferromagnetic ground state. We show that correlation effects render the hole and electron case in iridates very different. An added electron forms a spin polaron, similar to the cuprates, but the situation of a removed electron is far more complex. Many-body 5d 4 configurations form which can be singlet and triplet states of total angular momentum that strongly affect the hole motion. This not only has ramifications for the interpretation of (inverse-)photoemission experiments but also demonstrates that correlation physics renders electron- and hole-doped iridates fundamentally different.Some iridate compounds such as Sr 2 IrO 4 have electronic and atomic structures similar to quasi-2D copper oxides, raising the prospect of high temperature superconductivity. Here, the authors show that there is significant electron-hole asymmetry in iridates, contrary to expectations from the cuprates.

Early-type galaxy core phase densities

International Nuclear Information System (INIS)

Carlberg, R. G.; Hartwick, F. D. A.

2014-01-01

Early-type galaxies have projected central density brightness profile logarithmic slopes, γ', ranging from about 0 to 1. We show that γ' is strongly correlated, r = 0.83, with the coarse grain phase density of the galaxy core, Q 0 ≡ ρ/σ 3 . The luminosity-γ' correlation is much weaker, r = –0.51. Q 0 also serves to separate the distribution of steep core profiles, γ' > 0.5, from shallow profiles, γ' < 0.3, although there are many galaxies of intermediate slope, at intermediate Q 0 , in a volume-limited sample. The transition phase density separating the two profile types is approximately 0.003 M ☉ pc –3 km –3 s 3 , which is also where the relation between Q 0 and core mass shows a change in slope, the rotation rate of the central part of the galaxy increases, and the ratio of the black hole to core mass increases. These relations are considered relative to the globular cluster inspiral core buildup and binary black hole core scouring mechanisms for core creation and evolution. Mass-enhanced globular cluster inspiral models have quantitative predictions that are supported by data, but no single model yet completely explains the correlations.

Correlation effects on spin-polarized electron-hole quantum bilayer

Energy Technology Data Exchange (ETDEWEB)

Saini, L. K., E-mail: drlalitsaini75@gmail.com; Sharma, R. O., E-mail: sharmarajesh0387@gmail.com [Department of Applied Physics, S. V. National Institute of Technology, Surat – 395 007 (India); Nayak, Mukesh G. [Department of Physics, Silvassa College (Silvassa Institute of Higher Learning), Silvassa 396 230 (India)

2016-05-06

We present a numerical calculation for the intra- and interlayer pair-correlation functions, g{sub ll’}(r), of spin-polarized electron-hole quantum bilayers at zero temperature. The calculations of g{sub ll’}(r) are performed by including electron correlations within the dynamical version of the self-consistent mean-field approximation of Singwi, Tosi, Land and Sjölander (qSTLS). Our study reveals that the critical layer density decreases (increases) due to the inclusion of finite width (mass-asymmetry) effect during the phase-transition from charge-density wave to Wigner crystal ground-state by yielding the pronounced oscillatory behavior ing{sub ll}(r). The results are compared with recent findings of spin-polarized electron-hole quantum bilayers with mass-symmetry and zero width effects. To highlight the importance of dynamical character of correlations, we have also compared our results with the STLS results.

Influence of Nonfused Cores on the Photovoltaic Performance of Linear Triphenylamine-Based Hole-Transporting Materials for Perovskite Solar Cells.

Science.gov (United States)

Wu, Yungen; Wang, Zhihui; Liang, Mao; Cheng, Hua; Li, Mengyuan; Liu, Liyuan; Wang, Baiyue; Wu, Jinhua; Prasad Ghimire, Raju; Wang, Xuda; Sun, Zhe; Xue, Song; Qiao, Qiquan

2018-05-18

The core plays a crucial role in achieving high performance of linear hole transport materials (HTMs) toward the perovskite solar cells (PSCs). Most studies focused on the development of fused heterocycles as cores for HTMs. Nevertheless, nonfused heterocycles deserve to be studied since they can be easily synthesized. In this work, we reported a series of low-cost triphenylamine HTMs (M101-M106) with different nonfused cores. Results concluded that the introduced core has a significant influence on conductivity, hole mobility, energy level, and solubility of linear HTMs. M103 and M104 with nonfused oligothiophene cores are superior to other HTMs in terms of conductivity, hole mobility, and surface morphology. PSCs based on M104 exhibited the highest power conversion efficiency of 16.50% under AM 1.5 sun, which is comparable to that of spiro-OMeTAD (16.67%) under the same conditions. Importantly, the employment of M104 is highly economical in terms of the cost of synthesis as compared to that of spiro-OMeTAD. This work demonstrated that nonfused heterocycles, such as oligothiophene, are promising cores for high performance of linear HTMs toward PSCs.

Correlations among FBR core characteristics for various fuel compositions

International Nuclear Information System (INIS)

Maruyama, Shuhei; Ohki, Shigeo; Okubo, Tsutomu; Kawashima, Katsuyuki; Mizuno, Tomoyasu

2012-01-01

In the design of a fast breeder reactor (FBR) core for the light water reactor (LWR) to FBR transition stage, it is indispensable to grasp the effect of a wide range of fuel composition variations on the core characteristics. This study finds good correlations between burnup reactivity and safety parameters, such as the sodium void reactivity and Doppler coefficient, for various fuel compositions and determines the mechanisms behind these correlations with the aid of sensitivity analyses. It is clarified that the Doppler coefficient is actually correlated with the other core characteristics by considering the constraint imposed by the requirement of sustaining criticality on the fuel composition variations. These correlations make it easy to specify the various properties ranges for core reactivity control and core safety, which are important for core design in determining the core specifications and performance. They provide significant information for FBR core design for the transition stage. Moreover, as an application of the above-mentioned correlations, a simplified burnup reactivity index is developed for rapid and rational estimation of the core characteristic variations. With the use of this index and these correlations, the core characteristic variations can be estimated for various fuel compositions without repeating the core calculations. (author)

BLACK HOLE FORMATION IN FAILING CORE-COLLAPSE SUPERNOVAE

International Nuclear Information System (INIS)

O'Connor, Evan; Ott, Christian D.

2011-01-01

We present results of a systematic study of failing core-collapse supernovae and the formation of stellar-mass black holes (BHs). Using our open-source general-relativistic 1.5D code GR1D equipped with a three-species neutrino leakage/heating scheme and over 100 presupernova models, we study the effects of the choice of nuclear equation of state (EOS), zero-age main sequence (ZAMS) mass and metallicity, rotation, and mass-loss prescription on BH formation. We find that the outcome, for a given EOS, can be estimated, to first order, by a single parameter, the compactness of the stellar core at bounce. By comparing protoneutron star (PNS) structure at the onset of gravitational instability with solutions of the Tolman-Oppenheimer-Volkof equations, we find that thermal pressure support in the outer PNS core is responsible for raising the maximum PNS mass by up to 25% above the cold NS value. By artificially increasing neutrino heating, we find the critical neutrino heating efficiency required for exploding a given progenitor structure and connect these findings with ZAMS conditions, establishing, albeit approximately, for the first time based on actual collapse simulations, the mapping between ZAMS parameters and the outcome of core collapse. We also study the effect of progenitor rotation and find that the dimensionless spin of nascent BHs may be robustly limited below a* = Jc/GM 2 = 1 by the appearance of nonaxisymmetric rotational instabilities.

Ultrafast Transient Absorption Spectroscopy Investigation of Photoinduced Dynamics in Novel Donor-Acceptor Core-Shell Nanostructures for Organic Photovoltaics

Science.gov (United States)

Strain, Jacob; Jamhawi, Abdelqader; Abeywickrama, Thulitha M.; Loomis, Wendy; Rathnayake, Hemali; Liu, Jinjun

2016-06-01

Novel donor-acceptor nanostructures were synthesized via covalent synthesis and/or UV cross-linking method. Their photoinduced dynamics were investigated with ultrafast transient absorption (TA) spectroscopy. These new nanostructures are made with the strategy in mind to reduce manufacturing steps in the process of fabricating an organic photovoltaic cell. By imitating the heterojunction interface within a fixed particle domain, several fabrication steps can be bypassed reducing cost and giving more applicability to other film deposition methods. Such applications include aerosol deposition and ink-jet printing. The systems that were studied by TA spectroscopy include PDIB core, PDIB-P3HT core-shell, and PDIB-PANT core-shell which range in size from 60 to 130 nm. Within the experimentally accessible spectra range there resides a region of ground state bleaching, stimulated emission, and excited-state absorption of both neutrals and anions. Control experiments have been carried out to assign these features. At high pump fluences the TA spectra of PDIB core alone also indicate an intramolecular charge separation. The TA spectroscopy results thus far suggest that the core-shells resemble the photoinduced dynamics of a standard film although the particles are dispersed in solution, which indicates the desired outcome of the work.

Spectral hole-burning and carrier-heating dynamics in InGaAs quantum-dot amplifiers

DEFF Research Database (Denmark)

Borri, Paola; Langbein, Wolfgang Werner; Hvam, Jørn Märcher

2000-01-01

recovery of the spectral hole within ~100 fs is measured, comparable to bulk and quantum-well amplifiers, which is contradicting a carrier relaxation bottleneck in electrically pumped QD devices. The CH dynamics in the QD is quantitatively compared with results on an InGaAsP bulk amplifier. Reduced CH......The ultrafast gain and index dynamics in a set of InAs-InGaAs-GaAs quantum-dot (QD) amplifiers are measured at room temperature with femtosecond resolution. The role of spectral hole-burning (SHB) and carrier heating (CH) in the recovery of gain compression is investigated in detail. An ultrafast...

On the ultrafast charge migration and subsequent charge directed reactivity in Cl⋯N halogen-bonded clusters following vertical ionization

Energy Technology Data Exchange (ETDEWEB)

Chandra, Sankhabrata; Bhattacharya, Atanu, E-mail: atanub@ipc.iisc.ernet.in [Department of Inorganic and Physical Chemistry, Indian Institute of Science, Bangalore (India); Periyasamy, Ganga [Department of Chemistry, Central College Campus, Bangalore University, Bangalore (India)

2015-06-28

In this article, we have presented ultrafast charge transfer dynamics through halogen bonds following vertical ionization of representative halogen bonded clusters. Subsequent hole directed reactivity of the radical cations of halogen bonded clusters is also discussed. Furthermore, we have examined effect of the halogen bond strength on the electron-electron correlation- and relaxation-driven charge migration in halogen bonded complexes. For this study, we have selected A-Cl (A represents F, OH, CN, NH{sub 2}, CF{sub 3}, and COOH substituents) molecules paired with NH{sub 3} (referred as ACl:NH{sub 3} complex): these complexes exhibit halogen bonds. To the best of our knowledge, this is the first report on purely electron correlation- and relaxation-driven ultrafast (attosecond) charge migration dynamics through halogen bonds. Both density functional theory and complete active space self-consistent field theory with 6-31 + G(d, p) basis set are employed for this work. Upon vertical ionization of NCCl⋯NH{sub 3} complex, the hole is predicted to migrate from the NH{sub 3}-end to the ClCN-end of the NCCl⋯NH{sub 3} complex in approximately 0.5 fs on the D{sub 0} cationic surface. This hole migration leads to structural rearrangement of the halogen bonded complex, yielding hydrogen bonding interaction stronger than the halogen bonding interaction on the same cationic surface. Other halogen bonded complexes, such as H{sub 2}NCl:NH{sub 3}, F{sub 3}CCl:NH{sub 3}, and HOOCCl:NH{sub 3}, exhibit similar charge migration following vertical ionization. On the contrary, FCl:NH{sub 3} and HOCl:NH{sub 3} complexes do not exhibit any charge migration following vertical ionization to the D{sub 0} cation state, pointing to interesting halogen bond strength-dependent charge migration.

An ultrasensitive electrochemical biosensor for glucose using CdTe-CdS core-shell quantum dot as ultrafast electron transfer relay between graphene-gold nanocomposite and gold nanoparticle

International Nuclear Information System (INIS)

Gu Zhiguo; Yang Shuping; Li Zaijun; Sun Xiulan; Wang Guangli; Fang Yinjun; Liu Junkang

2011-01-01

Graphical abstract: We first reported an ultrasensitive electrochemical biosensor for glucose using CdTe-CdS core-shell quantum dot as ultrafast electron transfer relay between graphene-gold nanocomposite and gold nanoparticle. Since promising their electrocatalytic synergy towards glucose was achieved, the biosensor showed high sensitivity (5762.8 nA nM -1 cm -2 ), low detection limit (S/N = 3) (3 x 10 -12 M) and fast response time (0.045 s). - Abstract: The paper reported an ultrasensitive electrochemical biosensor for glucose which was based on CdTe-CdS core-shell quantum dot as ultrafast electron transfer relay between graphene-gold nanocomposite and gold nanoparticle. Since efficient electron transfer between glucose oxidase and the electrode was achieved, the biosensor showed high sensitivity (5762.8 nA nM -1 cm -2 ), low detection limit (S/N = 3) (3 x 10 -12 M), fast response time (0.045 s), wide calibration range (from 1 x 10 -11 M to 1 x 10 -8 M) and good long-term stability (26 weeks). The apparent Michaelis-Menten constant of the glucose oxidase on the medium, 5.24 x 10 -6 mM, indicates excellent bioelectrocatalytic activity of the immobilized enzyme towards glucose oxidation. Moreover, the effects of omitting graphene-gold nanocomposite, CdTe-CdS core-shell quantum dot and gold nanoparticle were also investigated. The result showed sensitivity of the biosensor is 7.67-fold better if graphene-gold nanocomposite, CdTe-CdS core-shell quantum dot and gold nanoparticle are used. This could be ascribed to improvement of the conductivity between graphene nanosheets due to introduction of gold nanoparticles, ultrafast charge transfer from CdTe-CdS core-shell quantum dot to graphene nanosheets and gold nanoparticle due to unique electrochemical properties of the CdTe-CdS core-shell quantum dot and good biocompatibility of gold nanoparticle for glucose oxidase. The biosensor is of best sensitivity in all glucose biosensors based on graphene nanomaterials up to

An ultrasensitive electrochemical biosensor for glucose using CdTe-CdS core-shell quantum dot as ultrafast electron transfer relay between graphene-gold nanocomposite and gold nanoparticle

Energy Technology Data Exchange (ETDEWEB)

Gu Zhiguo; Yang Shuping [School of Chemical and Material Engineering, Jiangnan University, Wuxi 214122 (China); Li Zaijun, E-mail: zaijunli@263.net [School of Chemical and Material Engineering, Jiangnan University, Wuxi 214122 (China); Sun Xiulan [School of Food Science and Technology, Jiangnan University, Wuxi 214122 (China); Wang Guangli [School of Chemical and Material Engineering, Jiangnan University, Wuxi 214122 (China); Fang Yinjun [Zhejiang Zanyu Technology Co., Ltd., Hangzhou 310009 (China); Liu Junkang [School of Chemical and Material Engineering, Jiangnan University, Wuxi 214122 (China)

2011-10-30

Graphical abstract: We first reported an ultrasensitive electrochemical biosensor for glucose using CdTe-CdS core-shell quantum dot as ultrafast electron transfer relay between graphene-gold nanocomposite and gold nanoparticle. Since promising their electrocatalytic synergy towards glucose was achieved, the biosensor showed high sensitivity (5762.8 nA nM{sup -1} cm{sup -2}), low detection limit (S/N = 3) (3 x 10{sup -12} M) and fast response time (0.045 s). - Abstract: The paper reported an ultrasensitive electrochemical biosensor for glucose which was based on CdTe-CdS core-shell quantum dot as ultrafast electron transfer relay between graphene-gold nanocomposite and gold nanoparticle. Since efficient electron transfer between glucose oxidase and the electrode was achieved, the biosensor showed high sensitivity (5762.8 nA nM{sup -1} cm{sup -2}), low detection limit (S/N = 3) (3 x 10{sup -12} M), fast response time (0.045 s), wide calibration range (from 1 x 10{sup -11} M to 1 x 10{sup -8} M) and good long-term stability (26 weeks). The apparent Michaelis-Menten constant of the glucose oxidase on the medium, 5.24 x 10{sup -6} mM, indicates excellent bioelectrocatalytic activity of the immobilized enzyme towards glucose oxidation. Moreover, the effects of omitting graphene-gold nanocomposite, CdTe-CdS core-shell quantum dot and gold nanoparticle were also investigated. The result showed sensitivity of the biosensor is 7.67-fold better if graphene-gold nanocomposite, CdTe-CdS core-shell quantum dot and gold nanoparticle are used. This could be ascribed to improvement of the conductivity between graphene nanosheets due to introduction of gold nanoparticles, ultrafast charge transfer from CdTe-CdS core-shell quantum dot to graphene nanosheets and gold nanoparticle due to unique electrochemical properties of the CdTe-CdS core-shell quantum dot and good biocompatibility of gold nanoparticle for glucose oxidase. The biosensor is of best sensitivity in all glucose

The Effect of the Holes Size Change of Lower-Support-Structure-Bottom Plate on the Reactor Core-Inlet Flow-Distribution

International Nuclear Information System (INIS)

Lee, Gong Hee; Bang, Young Seok; Cheong, Ae Ju

2015-01-01

Complex thermal-hydraulic phenomena exist inside PWR because reactor interiors include a fuel assembly, control rod assembly, ICI (In-Core Instrumentation), and other internal structures. Because changes to reactor design may influence interior, thermal-hydraulic characteristics, licensing applicants commonly conduct a flow-distribution test and use test results (e.g., core-inlet flow-rate distribution) as the input data for a core thermal-margin analysis program. Because the APR+ (Advanced Power Reactor Plus) had more fuel assemblies (241EA → 257EA) and the design of some internal structures was changed (from those of APR1400), the core-inlet flow-rate distribution for a 1/5 scaled-down reactor model was measured and high flow-rates were found especially near the outer region of the reactor core. In this study, to examine the effect of the holes size change (i.e. smaller diameter) in the outer region of the LSSBP, not a 50% blockage of the flow holes, on the reactor core-inlet flow-distribution, simulations were conducted with the commercial CFD (Computational Fluid Dynamics) software, ANSYS CFX R.14. The predicted results were compared with those of the original LSSBP. In this study, to examine the effect of the holes size change (smaller diameter) in the outer region of the LSSBP on the reactor core-inlet flow-distribution, simulations were conducted with the commercial CFD software, ANSYS CFX R.14. The predicted results were compared with those of the original LSSBP. Through these comparisons it was concluded that a more uniform distribution of the mass-flow rate at the core-inlet plane could be obtained by reducing the holes size in the outer region of the LSSBP

Developing standardized connection analysis techniques for slim hole core rod designs

International Nuclear Information System (INIS)

Fehr, G.; Bailey, E.I.

1994-01-01

Slim hole core rod design remains essentially in the proprietary domain. API standardization provides the ability to perform engineering analyses and dimensional inspections through the use of documents, ie: Specifications, Bulletins, and Recommended Practices. In order to provide similar engineering capability for non-API slim hole connections, this paper develops the initial phase of what may evolve into an engineering tool to provide at least an indication of relative serviceability between two connection styles for a given application. The starting point for this process will look at bending strength ratios and connection strength calculations. Since empirical data are yet needed to verify the approaches proposed in this paper, it is recognized that the alternatives presented here are only a first step to developing useful rules of thumb which may lead to later standardization

Dynamical effects of electron-hole correlation and giant quantum attenuation of ultrasound in semimetals

International Nuclear Information System (INIS)

Kuramoto, Y.

1982-01-01

The giant quantum attenuation of ultrasound in bismuth and other semimetals is noticeably enhanced when certain pair of Landau subbands of electrons and holes participate simultaneously in an attenuation peak. A theoretical analysis is presented which emphasizes importance of dynamical effects of the electron-hole correlation. In the temperature range between 1K and 4K covered by most experiments, the correlation effect is found to be weak on the real part of the relevant response function which gives change in sound velocity. This implies that equilibrium properties of the system are not much influenced by the correlation effect. Nonetheless, the electron-hole correlation is shown to have a drastic consequence on the imaginary part of the response function probed by the ultrasonic attenuation. Proposal for experiment is advanced to discriminate relative importance of this exciton-like correlation from that of repulsive correlation between carriers with the same charge. (orig.)

Core-hole effects in the x-ray-absorption spectra of transition-metal silicides

NARCIS (Netherlands)

WEIJS, PJW; CZYZYK, MT; VANACKER, JF; SPEIER, W; GOEDKOOP, JB; VANLEUKEN, H; HENDRIX, HJM; DEGROOT, RA; VANDERLAAN, G; BUSCHOW, KHJ; WIECH, G; FUGGLE, JC

1990-01-01

We report systematic differences between the shape of the Si K x-ray-absorption spectra of transition-metal silicides and broadened partial densities of Si p states. We use a variety of calculations to show that the origin of these discrepancies is the core-hole potential appropriate to the final

Preliminary petrographic and geophysical interpretations of the exploratory geothermal drill hole and core, Redstone, New Hampshire

Energy Technology Data Exchange (ETDEWEB)

Hoag, R.B. Jr.; Stewart, G.W.

1977-06-30

A 3000 foot diamond drill hole was drilled in the Conway Granite in Redstone, New Hampshire. A comprehensive detailed petrographic and physical study of this core was made. The purpose of this study is to supply a sound data base for future geothermal and uranium-thorium studies of the drill core. An estimate of the heat flow potential of the Redstone drill hole gives a heat flow of 1.9 HFU. If only the red phase of the Conway Granite had been intersected the heat flow may have been as much as 2.7 HFU, reaching a temperature of 260/sup 0/C at 6 km. The drill hole intersected four lithologies; the green and red phase of the Conway Granite, the Albany quartz syenite and a medium-grained, hastingsite-biotite granite. The red phase has the highest and most irregular radioactivity. The irregularity is mainly due to minor variations in lithology. The drill core intersected several alteration zones up to a thickness of 150 feet. These alteration zones represent passage of low to medium temperature fluids which might have been mineralized. The Conway Granite has the physical and chemical characteristics necessary for the formation of vein type uranium deposits. The presence of unexplained radiometric anomalies lends support to the existence of such deposits.

Electronic correlations in hole- and electron-doped Fe-based superconductors

Science.gov (United States)

Hardy, Frederic; Boehmer, Anna; Schweiss, Peter; Wolf, Thomas; Heid, Rolf; Eder, Robert; Fisher, Robert A.; Meingast, Christoph

2015-03-01

High-temperature superconductivity in the cuprates occurs at the crossover from a highly-correlated Mott insulating state to a weaker correlated Fermi liquid as a function of hole doping. The iron pnictides were initially thought to be fairly weakly correlated. However, we have recently shown using transport and thermodynamic measurements that KFe2As2 is strongly correlated. Both the Sommerfeld coefficient and the Pauli susceptibility are strongly enhanced with respect to their bare DFT values. These correlations are even further enhanced in RbFe2As2andCsFe2As2. The temperature dependence of both the susceptibility and the thermal expansion provides strong experimental evidence for the existence of a coherence-incoherence crossover; similar to what is found in heavy-fermion compounds. Whereas the correlations in the cuprates result from a large value of the Hubbard U, recent works have stressed the particular relevance of Hund's coupling in the pnictides. Our data may be interpreted in terms of a close proximity of KFe2As2 to an orbital-selective Mott transition. We now have good thermodynamic data covering both the hole and electron sides of the BaFe2As2 system and we will discuss how these correlations are modified by doping.

Modeling Polarized Emission from Black Hole Jets: Application to M87 Core Jet

Directory of Open Access Journals (Sweden)

Monika Mościbrodzka

2017-09-01

Full Text Available We combine three-dimensional general-relativistic numerical models of hot, magnetized Advection Dominated Accretion Flows around a supermassive black hole and the corresponding outflows from them with a general relativistic polarized radiative transfer model to produce synthetic radio images and spectra of jet outflows. We apply the model to the underluminous core of M87 galaxy. The assumptions and results of the calculations are discussed in context of millimeter observations of the M87 jet launching zone. Our ab initio polarized emission and rotation measure models allow us to address the constrains on the mass accretion rate onto the M87 supermassive black hole.

Correlation of transmissive fractures in pilot holes ONK-PH8 - PH12 and fracture traces mapped in ONKALO

International Nuclear Information System (INIS)

Palmen, J.; Nummela, J.; Ahokas, H.

2014-05-01

In a preceding study Posiva flow logging (PFL) with a 0.5 m test interval and 0.1 m steps has been used together with optical drillhole images and core logging fracture data for the exact determination of the depth of hydraulically conductive fractures in pilot holes. The fracture traces have been mapped from the ONKALO tunnel walls as a part of the systematic mapping. The mapping results has been digitized to a 3D tunnel layout in Surpac programme. The data integrity and fracture trace uniqueness has been verified by Datactica Oy and further collected to a database (RakokantaDatacticaPosiva20100607.mdb). Fractures mapped with leakage attribute have been defined as flowing, dripping, wet, or damp where the attribute is recorded. The fractures with no leakage attribute value appear to be non leaking. The water leaking surfaces on the ONKALO tunnel walls have been mapped sequentially and conclusively (once or twice a year) as a part of the Olkiluoto monitoring program (OMO) using an equal five step measure as used with fracture traces in systematic mapping. The PFL results correlated with core logging fracture data from the pilot holes ONK-PH8 - ONK-PH12 were in this work further correlated with the fractures mapped from the ONKALO tunnel walls. Each hydraulically conductive fracture of ONK-PH8 - ONK-PH12 was investigated and linked to ONKALO fracture of a coherent orientation and matching location, where such fracture trace was available. Also tunnel crosscutting fracture (TCF) data was used in combining, since the systematic mapping data was not yet available for the pilot holes ONK-PH11 and ONK-PH12 at the time of the evaluation. The main objective of the work was to identify the ONKALO fractures which correspond to the flow from fracture(s) identified with the PFL method in pilot holes and to collect basic information about the occurrence, frequency and orientation of water bearing fractures along the ONKALO tunnel. The correlated hydraulically conductive

Correlation of transmissive fractures in pilot holes ONK-PH8 - PH12 and fracture traces mapped in ONKALO

Energy Technology Data Exchange (ETDEWEB)

Palmen, J.; Nummela, J.; Ahokas, H. [Poeyry Finland Oy, Vantaa (Finland)

2014-05-15

In a preceding study Posiva flow logging (PFL) with a 0.5 m test interval and 0.1 m steps has been used together with optical drillhole images and core logging fracture data for the exact determination of the depth of hydraulically conductive fractures in pilot holes. The fracture traces have been mapped from the ONKALO tunnel walls as a part of the systematic mapping. The mapping results has been digitized to a 3D tunnel layout in Surpac programme. The data integrity and fracture trace uniqueness has been verified by Datactica Oy and further collected to a database (RakokantaDatacticaPosiva20100607.mdb). Fractures mapped with leakage attribute have been defined as flowing, dripping, wet, or damp where the attribute is recorded. The fractures with no leakage attribute value appear to be non leaking. The water leaking surfaces on the ONKALO tunnel walls have been mapped sequentially and conclusively (once or twice a year) as a part of the Olkiluoto monitoring program (OMO) using an equal five step measure as used with fracture traces in systematic mapping. The PFL results correlated with core logging fracture data from the pilot holes ONK-PH8 - ONK-PH12 were in this work further correlated with the fractures mapped from the ONKALO tunnel walls. Each hydraulically conductive fracture of ONK-PH8 - ONK-PH12 was investigated and linked to ONKALO fracture of a coherent orientation and matching location, where such fracture trace was available. Also tunnel crosscutting fracture (TCF) data was used in combining, since the systematic mapping data was not yet available for the pilot holes ONK-PH11 and ONK-PH12 at the time of the evaluation. The main objective of the work was to identify the ONKALO fractures which correspond to the flow from fracture(s) identified with the PFL method in pilot holes and to collect basic information about the occurrence, frequency and orientation of water bearing fractures along the ONKALO tunnel. The correlated hydraulically conductive

Residual stress measurement of PMMA by combining drilling-hole with digital speckle correlation method

Science.gov (United States)

Yao, X. F.; Xiong, T. C.; Xu, H. M.; Wan, J. P.; Long, G. R.

2008-11-01

The residual stresses of the PMMA (polymethyl methacrylate) specimens after being drilled, reamed and polished respectively are investigated using the digital speckle correlation experimental method,. According to the displacement fields around the correlated calculated region, the polynomial curve fitting method is used to obtain the continuous displacement fields, and the strain fields can be obtained from the derivative of the displacement fields. Considering the constitutive equation of the material, the expression of the residual stress can be presented. During the data processing, according to the fitting effect of the data, the calculation region of the correlated speckles and the degree of the polynomial fitting curve is decided. These results show that the maximum stress is at the hole-wall of the drilling hole specimen and with the increasing of the diameter of the drilled hole, the residual stress resulting from the hole drilling increases, whereas the process of reaming and polishing hole can reduce the residual stress. The relative large discrete degree of the residual stress is due to the chip removal ability of the drill bit, the cutting feed of the drill and other various reasons.

Preliminary analysis of geophysical logs from drill hole UE-25p No. 1, Yucca Mountain, Nye County, Nevada

International Nuclear Information System (INIS)

Muller, D.C.; Kibler, J.E.

1984-01-01

Geophysical logs from drill hole UE-25p No. 1 correlate well with logs through the same geologic units from other drill holes at Yucca Mountain, Nevada. The in-situ physical properties of the rocks as determined from well logs are consistent with laboratory-measured physical properties of core from other drill holes. The density, neutron and caliper logs are very spiky through most of the Topopah Spring Member. This spikiness occurs on the same logs in cored holes where the Topopah Spring Member is highly fractured and lithophysal. The uranium channel of the spectral gamma-ray log through the Topopah Spring Member correlates with uranium logs from cored holes where most of the fractures have not been healed or filled with materials that concentrate uranium. Therefore, fracture porosity and permeability of the Topopah Spring Member are expected to be high and consistent with fracture analysis from other drill holes on Yucca Mountain, and hydrologic tests from well J-13. The Paleozoic dolomites which underlie the Tertiary tuffs are intensely brecciated, and the uranium count rate is much higher than normal for dolomites because uranium has been concentrated in the recementing material. 19 references, 1 figure, 2 tables

Many-body correlation effects in the spatially separated electron and hole layers in the coupled quantum wells

Energy Technology Data Exchange (ETDEWEB)

Babichenko, V.S. [RRC Kurchatov Institute, Kurchatov Sq., 1, 123182 Moscow (Russian Federation); Polishchuk, I.Ya., E-mail: iyppolishchuk@gmail.com [RRC Kurchatov Institute, Kurchatov Sq., 1, 123182 Moscow (Russian Federation); Moscow Institute of Physics and Technology, 141700, 9, Institutskii per., Dolgoprudny, Moscow Region (Russian Federation)

2014-11-15

The many-body correlation effects in the spatially separated electron and hole layers in the coupled quantum wells are investigated. A special case of the many-component electron–hole system is considered. It is shown that if the hole mass is much greater than the electron mass, the negative correlation energy is mainly determined by the holes. The ground state of the system is found to be the 2D electron–hole liquid with the energy smaller than the exciton phase. It is shown that the system decays into the spatially separated neutral electron–hole drops if the initially created charge density in the layers is smaller than the certain critical value n{sub eq}.

Photonic crystal fiber technology for compact fiber-delivered high-power ultrafast fiber lasers

Science.gov (United States)

Triches, Marco; Michieletto, Mattia; Johansen, Mette M.; Jakobsen, Christian; Olesen, Anders S.; Papior, Sidsel R.; Kristensen, Torben; Bondue, Magalie; Weirich, Johannes; Alkeskjold, Thomas T.

2018-02-01

Photonic crystal fiber (PCF) technology has radically impacted the scientific and industrial ultrafast laser market. Reducing platform dimensions are important to decrease cost and footprint while maintaining high optical efficiency. We present our recent work on short 85 μm core ROD-type fiber amplifiers that maintain single-mode performance and excellent beam quality. Robust long-term performance at 100 W average power and 250 kW peak power in 20 ps pulses at 1030 nm wavelength is presented, exceeding 500 h with stable performance in terms of both polarization and power. In addition, we present our recent results on hollow-core ultrafast fiber delivery maintaining high beam quality and polarization purity.

ON THE ROLE OF FAST MAGNETIC RECONNECTION IN ACCRETING BLACK HOLE SOURCES

International Nuclear Information System (INIS)

Singh, C. B.; De Gouveia Dal Pino, E. M.; Kadowaki, L. H. S.

2015-01-01

We attempt to explain the observed radio and gamma-ray emission produced in the surroundings of black holes by employing a magnetically dominated accretion flow model and fast magnetic reconnection triggered by turbulence. In earlier work, a standard disk model was used and we refine the model by focusing on the sub-Eddington regime to address the fundamental plane of black hole activity. The results do not change substantially with regard to previous work, ensuring that the details of accretion physics are not relevant in the magnetic reconnection process occurring in the corona. Rather, our work puts fast magnetic reconnection events as a powerful mechanism operating in the core region near the jet base of black hole sources on more solid ground. For microquasars and low-luminosity active galactic nuclei, the observed correlation between radio emission and the mass of the sources can be explained by this process. The corresponding gamma-ray emission also seems to be produced in the same core region. On the other hand, emission from blazars and gamma-ray bursts cannot be correlated to core emission based on fast reconnection

Resolving ultrafast exciton migration in organic solids at the nanoscale

Science.gov (United States)

Ginsberg, Naomi

The migration of Frenkel excitons, tightly-bound electron-hole pairs, in photosynthesis and in organic semiconducting films is critical to the efficiency of natural and artificial light harvesting. While these materials exhibit a high degree of structural heterogeneity on the nanoscale, traditional measurements of exciton migration lengths are performed on bulk samples. Since both the characteristic length scales of structural heterogeneity and the reported bulk diffusion lengths are smaller than the optical diffraction limit, we adapt far-field super-resolution fluorescence imaging to uncover the correlations between the structural and energetic landscapes that the excitons explore. By combining the ultrafast super-resolved measurements with exciton hopping simulations we furthermore specify the nature (in addition to the extent) of exciton migration as a function of the intrinsic and ensemble chromophore energy scales that determine a spatio-energetic landscape for migration. In collaboration with: Samuel Penwell, Lucas Ginsberg, University of California, Berkeley and Rodrigo Noriega University of Utah.

Improving the clinical correlation of multiple sclerosis black hole volume change by paired-scan analysis.

Science.gov (United States)

Tam, Roger C; Traboulsee, Anthony; Riddehough, Andrew; Li, David K B

2012-01-01

The change in T 1-hypointense lesion ("black hole") volume is an important marker of pathological progression in multiple sclerosis (MS). Black hole boundaries often have low contrast and are difficult to determine accurately and most (semi-)automated segmentation methods first compute the T 2-hyperintense lesions, which are a superset of the black holes and are typically more distinct, to form a search space for the T 1w lesions. Two main potential sources of measurement noise in longitudinal black hole volume computation are partial volume and variability in the T 2w lesion segmentation. A paired analysis approach is proposed herein that uses registration to equalize partial volume and lesion mask processing to combine T 2w lesion segmentations across time. The scans of 247 MS patients are used to compare a selected black hole computation method with an enhanced version incorporating paired analysis, using rank correlation to a clinical variable (MS functional composite) as the primary outcome measure. The comparison is done at nine different levels of intensity as a previous study suggests that darker black holes may yield stronger correlations. The results demonstrate that paired analysis can strongly improve longitudinal correlation (from -0.148 to -0.303 in this sample) and may produce segmentations that are more sensitive to clinically relevant changes.

Uncertainty estimation of core safety parameters using cross-correlations of covariance matrix

International Nuclear Information System (INIS)

Yamamoto, A.; Yasue, Y.; Endo, T.; Kodama, Y.; Ohoka, Y.; Tatsumi, M.

2012-01-01

An uncertainty estimation method for core safety parameters, for which measurement values are not obtained, is proposed. We empirically recognize the correlations among the prediction errors among core safety parameters, e.g., a correlation between the control rod worth and assembly relative power of corresponding position. Correlations of uncertainties among core safety parameters are theoretically estimated using the covariance of cross sections and sensitivity coefficients for core parameters. The estimated correlations among core safety parameters are verified through the direct Monte-Carlo sampling method. Once the correlation of uncertainties among core safety parameters is known, we can estimate the uncertainty of a safety parameter for which measurement value is not obtained. Furthermore, the correlations can be also used for the reduction of uncertainties of core safety parameters. (authors)

PREFACE: Ultrafast biophotonics Ultrafast biophotonics

Science.gov (United States)

Gu, Min; Reid, Derryck; Ben-Yakar, Adela

2010-08-01

The use of light to explore biology can be traced to the first observations of tissue made with early microscopes in the mid-seventeenth century, and has today evolved into the discipline which we now know as biophotonics. This field encompasses a diverse range of activities, each of which shares the common theme of exploiting the interaction of light with biological material. With the rapid advancement of ultrafast optical technologies over the last few decades, ultrafast lasers have increasingly found applications in biophotonics, to the extent that the distinctive new field of ultrafast biophotonics has now emerged, where robust turnkey ultrafast laser systems are facilitating cutting-edge studies in the life sciences to take place in everyday laboratories. The broad spectral bandwidths, precision timing resolution, low coherence and high peak powers of ultrafast optical pulses provide unique opportunities for imaging and manipulating biological systems. Time-resolved studies of bio-molecular dynamics exploit the short pulse durations from such lasers, while other applications such as optical coherence tomography benefit from the broad optical bandwidths possible by using super-continuum generation and additionally allowing for high speed imaging with speeds as high as 47 000 scans per second. Continuing progress in laser-system technology is accelerating the adoption of ultrafast techniques across the life sciences, both in research laboratories and in clinical applications, such as laser-assisted in situ keratomileusis (LASIK) eye surgery. Revolutionizing the field of optical microscopy, two-photon excitation fluorescence (TPEF) microscopy has enabled higher spatial resolution with improved depth penetration into biological specimens. Advantages of this nonlinear optical process include: reduced photo-interactions, allowing for extensive imaging time periods; simultaneously exciting multiple fluorescent molecules with only one excitation wavelength; and

Feasibility of UltraFast Doppler in Post-operative Evaluation of Hepatic Artery in Recipients following Liver Transplantation.

Science.gov (United States)

Kim, Se-Young; Kim, Kyoung Won; Choi, Sang Hyun; Kwon, Jae Hyun; Song, Gi-Won; Kwon, Heon-Ju; Yun, Young Ju; Lee, Jeongjin; Lee, Sung-Gyu

2017-11-01

To determine the feasibility of using UltraFast Doppler in post-operative evaluation of the hepatic artery (HA) after liver transplantation (LT), we evaluated 283 simultaneous conventional and UltraFast Doppler sessions in 126 recipients over a 2-mo period after LT, using an Aixplorer scanner The Doppler indexes of the HA (peak systolic velocity [PSV], end-diastolic velocity [EDV], resistive index [RI] and systolic acceleration time [SAT]) by retrospective analysis of retrieved waves from UltraFast Doppler clips were compared with those obtained by conventional spectral Doppler. Correlation, performance in diagnosing the pathologic wave, examination time and reproducibility were evaluated. The PSV, EDV, RI and SAT of spectral and UltraFast Doppler measurements exhibited excellent correlation with favorable diagnostic performance. During the bedside examination, the mean time spent for UltraFast clip storing was significantly shorter than that for conventional Doppler US measurements. Both conventional and UltraFast Doppler exhibited good to excellent inter-analysis consistency. In conclusion, compared with conventional spectral Doppler, UltraFast Doppler values correlated excellently and yielded acceptable pathologic wave diagnostic performance with reduced examination time at the bedside and excellent reproducibility. Copyright © 2017 World Federation for Ultrasound in Medicine & Biology. Published by Elsevier Inc. All rights reserved.

Sediment cores from kettle holes in NE Germany reveal recent impacts of agriculture.

Science.gov (United States)

Kleeberg, Andreas; Neyen, Marielle; Schkade, Uwe-Karsten; Kalettka, Thomas; Lischeid, Gunnar

2016-04-01

Glacial kettle holes in young moraine regions receive abundant terrigenous material from their closed catchments. Core chronology and sediment accumulation were determined for two semi-permanent kettle holes, designated RG and KR, on arable land close to the villages of Rittgarten and Kraatz, respectively, in Uckermark, NE Germany. Core dating ((210)Pb, (137)Cs) revealed variable sediment accretion rates through time (RG 0.4-23.1 mm a(-1); KR 0.2-35.5 mm a(-1)), with periods of high accumulation corresponding to periods of intensive agricultural activity and consequent erosional inputs from catchments. Sediment composition (C, N, P, S, K, Ca, Fe, Mn, Zn, Cu, Mo, Pb, Cd, Zr) was used to determine sediment source and input processes. At RG, annual P input increased from 0.65 kg ha(-1) in the early nineteenth century to 1.67 kg ha(-1) by 2013. At KR, P input increased from 0.6 to 4.1 kg ha(-1) over the last century. There was a concurrent increase in Fe input in both water bodies. Thus, Fe/P ratios showed no temporal trend and did not differ between RG (18.5) and KR (18.4), indicating similar P mobility. At RG, the S/Fe ratio increased from 0.4 to 2.3, indicating more iron sulphides and thus higher P availability, coinciding with high coverage of duckweed (Spirodela polyrhiza (L.)) and soft hornwort (Ceratophyllum submersum L.). At KR, however, this ratio remained low and relatively unchanged (0.3 ± 0.4), indicating more efficient Fe-P binding and lower hydrophyte productivity. Trends in sediment composition indicate a shift towards eutrophication in both kettle holes, but with differences in timing and magnitude. Other morphologically similar kettle holes in NE Germany that are prone to erosion could have been similarly impacted but may differ in the extent of sediment infilling and degradation of their ecological functions.

NNWSI [Nevada Nuclear Waste Storage Investigations] hole histories: Unsaturated zone-neutron holes: 76 boreholes drilled between May 1984 and February 1986

International Nuclear Information System (INIS)

1987-05-01

This is a compilation of data from seventy-four shallow alluvial exploratory core holes and two shallow calibration core holes. The boreholes were drilled to obtain undisturbed alluvial cores, to determine vertical distribution of moisture content and water potential, and to run neutron moisture logs. Data presented in the hole histories include all locations, daily activities and review of hole conditions

A 17-billion-solar-mass black hole in a group galaxy with a diffuse core.

Science.gov (United States)

Thomas, Jens; Ma, Chung-Pei; McConnell, Nicholas J; Greene, Jenny E; Blakeslee, John P; Janish, Ryan

2016-04-21

Quasars are associated with and powered by the accretion of material onto massive black holes; the detection of highly luminous quasars with redshifts greater than z = 6 suggests that black holes of up to ten billion solar masses already existed 13 billion years ago. Two possible present-day 'dormant' descendants of this population of 'active' black holes have been found in the galaxies NGC 3842 and NGC 4889 at the centres of the Leo and Coma galaxy clusters, which together form the central region of the Great Wall--the largest local structure of galaxies. The most luminous quasars, however, are not confined to such high-density regions of the early Universe; yet dormant black holes of this high mass have not yet been found outside of modern-day rich clusters. Here we report observations of the stellar velocity distribution in the galaxy NGC 1600--a relatively isolated elliptical galaxy near the centre of a galaxy group at a distance of 64 megaparsecs from Earth. We use orbit superposition models to determine that the black hole at the centre of NGC 1600 has a mass of 17 billion solar masses. The spatial distribution of stars near the centre of NGC 1600 is rather diffuse. We find that the region of depleted stellar density in the cores of massive elliptical galaxies extends over the same radius as the gravitational sphere of influence of the central black holes, and interpret this as the dynamical imprint of the black holes.

Direct Characterization of Ultrafast Energy-Time Entangled Photon Pairs.

Science.gov (United States)

MacLean, Jean-Philippe W; Donohue, John M; Resch, Kevin J

2018-02-02

Energy-time entangled photons are critical in many quantum optical phenomena and have emerged as important elements in quantum information protocols. Entanglement in this degree of freedom often manifests itself on ultrafast time scales, making it very difficult to detect, whether one employs direct or interferometric techniques, as photon-counting detectors have insufficient time resolution. Here, we implement ultrafast photon counters based on nonlinear interactions and strong femtosecond laser pulses to probe energy-time entanglement in this important regime. Using this technique and single-photon spectrometers, we characterize all the spectral and temporal correlations of two entangled photons with femtosecond resolution. This enables the witnessing of energy-time entanglement using uncertainty relations and the direct observation of nonlocal dispersion cancellation on ultrafast time scales. These techniques are essential to understand and control the energy-time degree of freedom of light for ultrafast quantum optics.

Exciton and Hole-Transfer Dynamics in Polymer: Fullerene Blends

Directory of Open Access Journals (Sweden)

van Loosdrecht P. H. M.

2013-03-01

Full Text Available Ultrafast hole transfer dynamics from fullerene derivative to polymer in bulk heterojunction blends are studied with visible-pump - IR-probe spectroscopy. The hole transfer process is found to occur in 50/300 fs next to the interface, while a longer 15-ps time is attributed to exciton diffusion towards interface in PC71BM domains. High polaron generation efficiency in P3HT blends indicates excellent intercalation between the polymer and the fullerene even at highest PC71BM concentration thereby yielding a valuable information on the blend morphology.

Stabilized soliton self-frequency shift and 0.1- PHz sideband generation in a photonic-crystal fiber with an air-hole-modified core.

Science.gov (United States)

Liu, Bo-Wen; Hu, Ming-Lie; Fang, Xiao-Hui; Li, Yan-Feng; Chai, Lu; Wang, Ching-Yue; Tong, Weijun; Luo, Jie; Voronin, Aleksandr A; Zheltikov, Aleksei M

2008-09-15

Fiber dispersion and nonlinearity management strategy based on a modification of a photonic-crystal fiber (PCF) core with an air hole is shown to facilitate optimization of PCF components for a stable soliton frequency shift and subpetahertz sideband generation through four-wave mixing. Spectral recoil of an optical soliton by a red-shifted dispersive wave, generated through a soliton instability induced by high-order fiber dispersion, is shown to stabilize the soliton self-frequency shift in a highly nonlinear PCF with an air-hole-modified core relative to pump power variations. A fiber with a 2.3-microm-diameter core modified with a 0.9-microm-diameter air hole is used to demonstrate a robust soliton self-frequency shift of unamplified 50-fs Ti: sapphire laser pulses to a central wavelength of about 960 nm, which remains insensitive to variations in the pump pulse energy within the range from 60 to at least 100 pJ. In this regime of frequency shifting, intense high- and low-frequency branches of dispersive wave radiation are simultaneously observed in the spectrum of PCF output. An air-hole-modified-core PCF with appropriate dispersion and nonlinearity parameters is shown to provide efficient four-wave mixing, giving rise to Stokes and anti-Stokes sidebands whose frequency shift relative to the pump wavelength falls within the subpetahertz range, thus offering an attractive source for nonlinear Raman microspectroscopy.

Ultrafast dissociation: An unexpected tool for probing molecular dynamics

International Nuclear Information System (INIS)

Morin, Paul; Miron, Catalin

2012-01-01

Highlights: ► Ultrafast dissociation has been investigated by means of XPS and mass spectrometry. ► The interplay between electron relaxation and molecular dynamics is evidenced. ► Extension toward polyatomics, clusters, adsorbed molecules is considered. ► Quantum effects (spectral hole, angular effects) evidence the molecular field anisotropy. -- Abstract: Ultrafast dissociation following core–shell excitation into an antibonding orbital led to the early observation in HBr of atomic Auger lines associated to the decay of dissociated excited atoms. The purpose of this article is to review the very large variety of systems where such a situation has been encountered, extending from simple diatomic molecules toward more complex systems like polyatomics, clusters, or adsorbed molecules. Interestingly, this phenomenon has revealed an extremely rich and powerful tool for probing nuclear dynamics and its subtle interplay with electron relaxation occurring on a comparable time scale. Consequently this review covers a surprisingly large period, starting in 1986 and still ongoing.

Density of basalt core from Hilo drill hole, Hawaii

Science.gov (United States)

Moore, J.G.

2001-01-01

Density measurements of 1600 samples of core from 889 to 3097 m depth below sea level in the Hawaii Scientific Drilling Program hole near Hilo, Hawaii show marked differences between the basaltic rock types and help define stratigraphy in the hole. Water-saturated densities of subaerial lava flows (occurring above 1079 m depth) have the broadest range because of the large density variation within a single lava flow. Water-saturated densities commonly range from 2.0 to 3.0 with an average of 2.55 ?? 0.24 g/cc. Dikes and sills range from 2.8 to 3.1 g/cc). Densities of hyaloclastite commonly range from 2.3 to 2.7, with an overall average of about 2.5 g/cc. The low-density of most hyaloclastite is due primarily to palagonitization of abundant glass and presence of secondary minerals in the interstices between fragments. Four principal zones of pillow lava, separated by hyaloclastite, occur in the drill core. The shallowest (1983-2136 m) is paradoxically the densest, averaging 3.01 ?? 0.10 g/cc. The second (2234-2470 m) is decidedly the lightest, averaging 2.67 ?? 0.13 g/cc. The third (2640-2790 m) and fourth (2918-bottom at 3097 m) are high, averaging 2.89 ?? 0.17 and 2.97 ?? 0.08 g/cc, respectively. The first pillow zone includes degassed pillows i.e. lava erupted on land that flowed into the sea. These pillows are poor in vesicles, because the subaerial, one-atmosphere vesicles were compressed when the flow descended to deeper water and higher pressure. The second (low-density, non-degassed) pillow zone is the most vesicle-rich, apparently because it was erupted subaqueously at a shallow depth. The higher densities of the third and fourth zones result from a low vesicularity of only a few percent and an olivine content averaging more than 5% for the third zone and about 10% for the fourth zone. The uppermost hyaloclastite extending about 400 m below the bottom of the subaerial basalt is poorly cemented and absorbs up to 6 wt% of water when immersed. Progressing

Uncertainty estimation of core safety parameters using cross-correlations of covariance matrix

International Nuclear Information System (INIS)

Yamamoto, Akio; Yasue, Yoshihiro; Endo, Tomohiro; Kodama, Yasuhiro; Ohoka, Yasunori; Tatsumi, Masahiro

2013-01-01

An uncertainty reduction method for core safety parameters, for which measurement values are not obtained, is proposed. We empirically recognize that there exist some correlations among the prediction errors of core safety parameters, e.g., a correlation between the control rod worth and the assembly relative power at corresponding position. Correlations of errors among core safety parameters are theoretically estimated using the covariance of cross sections and sensitivity coefficients of core parameters. The estimated correlations of errors among core safety parameters are verified through the direct Monte Carlo sampling method. Once the correlation of errors among core safety parameters is known, we can estimate the uncertainty of a safety parameter for which measurement value is not obtained. (author)

GRAVITATIONAL WAVE SIGNATURES IN BLACK HOLE FORMING CORE COLLAPSE

Energy Technology Data Exchange (ETDEWEB)

Cerdá-Durán, Pablo; DeBrye, Nicolas; Aloy, Miguel A.; Font, José A.; Obergaulinger, Martin, E-mail: pablo.cerda@uv.es [Departamento de Astronomia y Astrofísica, Universidad de Valencia, c/Dr. Moliner 50, E-46100-Burjassot (Spain)

2013-12-20

We present general relativistic numerical simulations of collapsing stellar cores. Our initial model consists of a low metallicity rapidly-rotating progenitor which is evolved in axisymmetry with the latest version of our general relativistic code CoCoNuT, which allows for black hole formation and includes the effects of a microphysical equation of state (LS220) and a neutrino leakage scheme to account for radiative losses. The motivation of our study is to analyze in detail the emission of gravitational waves in the collapsar scenario of long gamma-ray bursts. Our simulations show that the phase during which the proto-neutron star (PNS) survives before ultimately collapsing to a black hole is particularly optimal for gravitational wave emission. The high-amplitude waves last for several seconds and show a remarkable quasi-periodicity associated with the violent PNS dynamics, namely during the episodes of convection and the subsequent nonlinear development of the standing-accretion shock instability (SASI). By analyzing the spectrogram of our simulations we are able to identify the frequencies associated with the presence of g-modes and with the SASI motions at the PNS surface. We note that the gravitational waves emitted reach large enough amplitudes to be detected with third-generation detectors such as the Einstein Telescope within a Virgo Cluster volume at rates ≲ 0.1 yr{sup –1}.

The fate of electron–hole pairs in polymer:fullerene blends for organic photovoltaics

KAUST Repository

Causa', Martina; Jonghe-Risse, Jelissa De; Scarongella, Mariateresa; Brauer, Jan C.; Domingo, Ester; Moser, Jacques-E.; Stingelin, Natalie; Banerji, Natalie

2016-01-01

demonstrate that the fate of photogenerated electron-hole pairs-whether they will dissociate to free charges or geminately recombine-is determined at ultrafast times, despite the fact that their actual spatial separation can be much slower. Our insights

Core-level photoemission revealing the Mott transition

International Nuclear Information System (INIS)

Kim, Hyeong-Do; Noh, Han-Jin; Kim, K.H.; Oh, S.-J.

2005-01-01

Ru 3d core-level X-ray photoemission spectra of various ruthenates are examined. They show in general two-peak structures, which can be assigned as the screened and unscreened peaks. The screened peak is absent in a Mott insulator, but develops into a main peak as the correlation strength becomes weak. This spectral behavior is well explained by the dynamical mean-field theory calculation for the single-band Hubbard model with the on-site core-hole potential using the exact diagonalization method. The new mechanism of the core-level photoemission satellite can be utilized to reveal the Mott transition phenomenon in various strongly correlated electron systems

Dynamical manifestations of quantum chaos: correlation hole and bulge

Science.gov (United States)

Torres-Herrera, E. J.; Santos, Lea F.

2017-10-01

A main feature of a chaotic quantum system is a rigid spectrum where the levels do not cross. We discuss how the presence of level repulsion in lattice many-body quantum systems can be detected from the analysis of their time evolution instead of their energy spectra. This approach is advantageous to experiments that deal with dynamics, but have limited or no direct access to spectroscopy. Dynamical manifestations of avoided crossings occur at long times. They correspond to a drop, referred to as correlation hole, below the asymptotic value of the survival probability and to a bulge above the saturation point of the von Neumann entanglement entropy and the Shannon information entropy. By contrast, the evolution of these quantities at shorter times reflects the level of delocalization of the initial state, but not necessarily a rigid spectrum. The correlation hole is a general indicator of the integrable-chaos transition in disordered and clean models and as such can be used to detect the transition to the many-body localized phase in disordered interacting systems. This article is part of the themed issue 'Breakdown of ergodicity in quantum systems: from solids to synthetic matter'.

Black holes in massive close binaries - observational data and evolutionary status

International Nuclear Information System (INIS)

Tutukov, A.V.; Cherepashchuk, A.M.; Moskovskii Gosudarstvennyi Universitet, Moscow, USSR)

1985-01-01

The available information on the mass of four candidate black holes in X-ray binary systems is summarized; these systems are compared with neutron star binaries with regard to the mass of their components. In mass, the relativistic objects form two distinct groups, neutron stars with masses equal to about 1-2 solar masses and black hole candidates with masses equal to about 10-60 solar masses (there seem to be no intermediate cases), but there is no correlation with the mass of the optical star. Mass exchange between the optical component of a close binary and its neutron star companion would be unlikely to produce a black hole more massive than 5-7 solar masses. Instead, the black holes having masses greater than about 10 solar masses might result from core collapse in stars of initial mass equating 20-100 solar masses through either a rise in the presupernova core mass or weakness of the magnetic field. The (10-30)-fold disparity in the incidence of black holes coupled with OB stars and with radio pulsars could indicate that black holes tend to form in pairs. 36 references

Correlation of transmissive fractures in holes OL-PH1, ONK-PH2 .. ONK-PH7 and ONKALO tunnel fractures

International Nuclear Information System (INIS)

Palmen, J; Nummela, J.; Ahokas, H.

2011-02-01

In a preceding study Posiva flow logging (PFL) with a 0.5 m test interval and 10 cm steps has been used together with optical drillhole images and core logging fracture data for the exact determination of the depth of hydraulically conductive fractures in pilot holes. The fracture traces has been mapped from the ONKALO tunnel walls as a part of the systematic mapping. The mapping results has been digitized to a 3D tunnel layout in Surpac Vision programme. The data integrity and fracture trace uniqueness has been verified by Datactica Oy and further collected to a database (Rakokanta D atactica P osiva20091119.mdb). Water leakage of the mapped fractures exists as an attribute field for each fracture, but the value of the attribute has not been assessed conclusively. Those fractures mapped with leakage attribute have been defined as flowing, dripping, wet, or damp where the attribute is recorded. The fractures with no leakage attribute value appear to be dry (not leaking) or the information is not available (assessment was not performed). The water leaking surfaces on ONKALO tunnel wall have been mapped sequentially and conclusively (twice a year) as a part of the Olkiluoto monitoring program (OMO) using an equal five step measure as used with fracture traces in systematic mapping. The PFL results correlated with core logging fracture data from pilot holes OL-PH1 and ONK-PH2 .. ONK-PH7 were in this work further correlated with the fractures mapped from the ONKALO tunnel walls. Each hydraulically conductive fracture of OL-PH1 and ONK-PH2 - ONK-PH7 was investigated and linked to ONKALO fracture of a coherent orientation and matching location, where such fracture trace was available. The main objective of the work was to identify the ONKALO fractures which correspond to the flow from fracture(s) identified with the PFL method in pilot holes and to collect basic information about the occurrence, frequency and orientation of water bearing fractures along ONKALO tunnel

Spin relaxation dynamics of holes in intrinsic GaAs quantum wells studied by transient circular dichromatic absorption spectroscopy at room temperature.

Science.gov (United States)

Fang, Shaoyin; Zhu, Ruidan; Lai, Tianshu

2017-03-21

Spin relaxation dynamics of holes in intrinsic GaAs quantum wells is studied using time-resolved circular dichromatic absorption spectroscopy at room temperature. It is found that ultrafast dynamics is dominated by the cooperative contributions of band filling and many-body effects. The relative contribution of the two effects is opposite in strength for electrons and holes. As a result, transient circular dichromatic differential transmission (TCD-DT) with co- and cross-circularly polarized pump and probe presents different strength at several picosecond delay time. Ultrafast spin relaxation dynamics of excited holes is sensitively reflected in TCD-DT with cross-circularly polarized pump and probe. A model, including coherent artifact, thermalization of nonthermal carriers and the cooperative contribution of band filling and many-body effects, is developed, and used to fit TCD-DT with cross-circularly polarized pump and probe. Spin relaxation time of holes is achieved as a function of excited hole density for the first time at room temperature, and increases with hole density, which disagrees with a theoretical prediction based on EY spin relaxation mechanism, implying that EY mechanism may be not dominant hole spin relaxation mechanism at room temperature, but DP mechanism is dominant possibly.

Delayed electron relaxation in CdTe nanorods studied by spectral analysis of the ultrafast transient absorption

International Nuclear Information System (INIS)

Kriegel, I.; Scotognella, F.; Soavi, G.; Brescia, R.; Rodríguez-Fernández, J.; Feldmann, J.; Lanzani, G.; Tassone, F.

2016-01-01

Highlights: • We study the photophysics of CdTe nanorods by ultrafast absorption spectroscopy. • We fit photobleaching and photoinduced absorption features at all time delays. • Dynamics are extracted from superpositions of bleaches (Gaussians) and derivatives. • Fast non-radiative recombination and slower hole trapping processes are extracted. • A potential approach to unveil ultrafast non-radiative recombination processes. - Abstract: In transient absorption (TA) spectra, the bleach features originating from state filling are overlapped by their energy-shifted derivatives, arising from excited state energy level shifts. This makes the direct extraction of carrier dynamics from a single-wavelength time-trace misleading. Fitting TA spectra in time, as Gaussian functions and their derivative-like shifted Gaussians, allows to individually extract the real dynamics of both photobleached transitions, and their energy shifts. In CdTe nanorods (NRs) we found a delayed heating of holes due to the release of the large excess energy in the electron relaxation process. The slow hole-trapping process is consistent with a high number of surface trap states in these model NRs. Our results show that only a correct disentanglement of bleaching and energy shift contributions provides a reliable framework to extract the underlying carrier relaxation dynamics, including trapping, non-radiative recombination, and eventually carrier multiplication.

Delayed electron relaxation in CdTe nanorods studied by spectral analysis of the ultrafast transient absorption

Energy Technology Data Exchange (ETDEWEB)

Kriegel, I., E-mail: ilka.kriegel@iit.it [Dipartimento di Fisica, Politecnico di Milano, Piazza Leonardo da Vinci 32, 20133 Milano (Italy); Scotognella, F. [Dipartimento di Fisica, Politecnico di Milano, Piazza Leonardo da Vinci 32, 20133 Milano (Italy); CNST of IIT@POLIMI, Via Pascoli 70/3, 20133 Milano (Italy); Soavi, G. [Dipartimento di Fisica, Politecnico di Milano, Piazza Leonardo da Vinci 32, 20133 Milano (Italy); Brescia, R. [Department of Nanochemistry, Istituto Italiano di Tecnologia (IIT), via Morego 30, 16163 Genova (Italy); Rodríguez-Fernández, J.; Feldmann, J. [Photonics and Optoelectronics Group, Department of Physics and CeNS, Ludwig-Maximilians-Universität München, Amalienstr. 54, 80799 Munich (Germany); Nanosystems Initiative Munich (NIM), Schellingstr. 4, 80799 Munich (Germany); Lanzani, G., E-mail: guglielmo.lanzani@iit.it [Dipartimento di Fisica, Politecnico di Milano, Piazza Leonardo da Vinci 32, 20133 Milano (Italy); CNST of IIT@POLIMI, Via Pascoli 70/3, 20133 Milano (Italy); Tassone, F. [CNST of IIT@POLIMI, Via Pascoli 70/3, 20133 Milano (Italy)

2016-06-01

Highlights: • We study the photophysics of CdTe nanorods by ultrafast absorption spectroscopy. • We fit photobleaching and photoinduced absorption features at all time delays. • Dynamics are extracted from superpositions of bleaches (Gaussians) and derivatives. • Fast non-radiative recombination and slower hole trapping processes are extracted. • A potential approach to unveil ultrafast non-radiative recombination processes. - Abstract: In transient absorption (TA) spectra, the bleach features originating from state filling are overlapped by their energy-shifted derivatives, arising from excited state energy level shifts. This makes the direct extraction of carrier dynamics from a single-wavelength time-trace misleading. Fitting TA spectra in time, as Gaussian functions and their derivative-like shifted Gaussians, allows to individually extract the real dynamics of both photobleached transitions, and their energy shifts. In CdTe nanorods (NRs) we found a delayed heating of holes due to the release of the large excess energy in the electron relaxation process. The slow hole-trapping process is consistent with a high number of surface trap states in these model NRs. Our results show that only a correct disentanglement of bleaching and energy shift contributions provides a reliable framework to extract the underlying carrier relaxation dynamics, including trapping, non-radiative recombination, and eventually carrier multiplication.

Observation of a cavitation cloud in tissue using correlation between ultrafast ultrasound images.

Science.gov (United States)

Prieur, Fabrice; Zorgani, Ali; Catheline, Stefan; Souchon, Rémi; Mestas, Jean-Louis; Lafond, Maxime; Lafon, Cyril

2015-07-01

The local application of ultrasound is known to improve drug intake by tumors. Cavitating bubbles are one of the contributing effects. A setup in which two ultrasound transducers are placed confocally is used to generate cavitation in ex vivo tissue. As the transducers emit a series of short excitation bursts, the evolution of the cavitation activity is monitored using an ultrafast ultrasound imaging system. The frame rate of the system is several thousands of images per second, which provides several tens of images between consecutive excitation bursts. Using the correlation between consecutive images for speckle tracking, a decorrelation of the imaging signal appears due to the creation, fast movement, and dissolution of the bubbles in the cavitation cloud. By analyzing this area of decorrelation, the cavitation cloud can be localized and the spatial extent of the cavitation activity characterized.

Variations of current profiles in tokamaks. Formation mechanism and confinement property of current-hole configuration

International Nuclear Information System (INIS)

Takizuka, Tomonori

2003-01-01

The formation mechanism of the current hole in tokamak plasmas is reviewed. Experimental results of JT-60U are shown. Increase of the off-central noninductive current is a key factor for the current-hole formation. The internal Transport Barrier (ITB), which generates large bootstrap current, plays an important role. The central current density in the hole stays nearly 0. The idea of a new equilibrium for a tokamak plasma with a current hole is introduced. This equilibrium configuration called Axisymmetric Tri-Magnetic-Islands (ATMI) equilibrium', has three islands along the R direction (a central-negative-current island and side-positive-current islands). The equilibrium is stable with the elongation coils when the current in the ATMI region is limited to a small amount. The confinement properties of a current-hole configuration with box-type ITB is described. A scaling of the core poloidal beta inside the ITB, β p,core , is given as ε f β p,core approx. = 1, which suggests the equilibrium limit (ε f : inverse aspect ratio at the ITB foot). Though the core stored energy is little dependent on the heating power, the estimated heat diffusivity in the ITB region moderately correlates with a neoclassical diffusivity. (author)

Radio transients from newborn black holes

Science.gov (United States)

Kashiyama, Kazumi; Hotokezaka, Kenta; Murase, Kohta

2018-05-01

We consider radio emission from a newborn black hole (BH), which is accompanied by a mini-disk with a mass of ≲ M⊙. Such a disk can be formed from an outer edge of the progenitor's envelope, especially for metal-poor massive stars and/or massive stars in close binaries. The disk accretion rate is typically super-Eddington and an ultrafast outflow with a velocity of ˜0.1-0.3 c will be launched into the circumstellar medium. The outflow forms a collisionless shock, and electrons are accelerated and emit synchrotron emission in radio bands with a flux of ˜ 10^{26-30} erg s^{-1} Hz^{-1} days to decades after the BH formation. The model predicts not only a fast UV/optical transient but also quasi-simultaneous inverse-Compton X-ray emission ˜ a few days after the BH formation, and the discovery of the radio counterpart with coordinated searches will enable us to identify this type of transients. The occurrence rate can be 0.1 - 10 % of the core-collapse supernova rate, which makes them a promising target of dedicated radio observations such as the Jansky VLA Sky Survey.

Oxygen 1s excitation and tetragonal distortion from core-hole effect in BaTiO3

Science.gov (United States)

Bugnet, Matthieu; Radtke, Guillaume; Botton, Gianluigi A.

2013-11-01

The accurate description of the O 1s excitation in BaTiO3 has been elusive so far. In this Rapid Communication, the electronic structure and the high-resolution electron energy-loss near-edge structures of the O K edge in tetragonal BaTiO3 are investigated using first-principles calculations. The results demonstrate a clear correlation between the broadening of the lower energy fine structure and the anisotropic effects induced by the core-hole potential, which are directly related to the structural distortion occurring in tetragonal BaTiO3. Moreover, we show that a significant improvement of the description of higher-lying structures can be obtained when correcting the energy position of the Ba 4f states. This demonstrates that the O 1s spectrum can be a very effective probe of the distortion and changes in the local electronic structure, and be used as a sensitive tool for studying new materials and ferroelectric transitions.

Supermassive Black Holes and their Host Spheroids III. The Mbh-nsph Correlation

Science.gov (United States)

Savorgnan, Giulia A. D.

2016-04-01

The Sérsic {R}1/n model is the best approximation known to date for describing the light distribution of stellar spheroidal and disk components, with the Sérsic index n providing a direct measure of the central radial concentration of stars. The Sérsic index of a galaxy’s spheroidal component, nsph, has been shown to tightly correlate with the mass of the central supermassive black hole, MBH. The {M}{BH}{--}{n}{sph} correlation is also expected from other two well known scaling relations involving the spheroid luminosity, Lsph: the {L}{sph}{--}{n}{sph} and the {M}{BH}{--}{L}{sph}. Obtaining an accurate estimate of the spheroid Sérsic index requires a careful modeling of a galaxy’s light distribution and some studies have failed to recover a statistically significant {M}{BH}{--}{n}{sph} correlation. With the aim of re-investigating the {M}{BH}{--}{n}{sph} and other black hole mass scaling relations, we performed a detailed (I.e., bulge, disks, bars, spiral arms, rings, halo, nucleus, etc.) decomposition of 66 galaxies, with directly measured black hole masses, that had been imaged at 3.6 μm with Spitzer. In this paper, the third of this series, we present an analysis of the {L}{sph}{--}{n}{sph} and {M}{BH}{--}{n}{sph} diagrams. While early-type (elliptical+lenticular) and late-type (spiral) galaxies split into two separate relations in the {L}{sph}{--}{n}{sph} and {M}{BH}{--}{L}{sph} diagrams, they reunite into a single {M}{BH}\\propto {n}{sph}3.39+/- 0.15 sequence with relatively small intrinsic scatter (ɛ ≃ 0.25 {dex}). The black hole mass appears to be closely related to the spheroid central concentration of stars, which mirrors the inner gradient of the spheroid gravitational potential.

BLACK HOLE-GALAXY CORRELATIONS WITHOUT SELF-REGULATION

International Nuclear Information System (INIS)

Anglés-Alcázar, Daniel; Özel, Feryal; Davé, Romeel

2013-01-01

Recent models of black hole growth in a cosmological context have forwarded a paradigm in which the growth is self-regulated by feedback from the black hole itself. Here we use cosmological zoom simulations of galaxy formation down to z = 2 to show that such strong self-regulation is required in the popular spherical Bondi accretion model, but that a plausible alternative model in which black hole growth is limited by galaxy-scale torques does not require self-regulation. Instead, this torque-limited accretion model yields black holes and galaxies evolving on average along the observed scaling relations by relying only on a fixed, 5% mass retention rate onto the black hole from the radius at which the accretion flow is fed. Feedback from the black hole may (and likely does) occur, but does not need to couple to galaxy-scale gas in order to regulate black hole growth. We show that this result is insensitive to variations in the initial black hole mass, stellar feedback, or other implementation details. The torque-limited model allows for high accretion rates at very early epochs (unlike the Bondi case), which if viable can help explain the rapid early growth of black holes, while by z ∼ 2 it yields Eddington factors of ∼1%-10%. This model also yields a less direct correspondence between major merger events and rapid phases of black hole growth. Instead, growth is more closely tied to cosmological disk feeding, which may help explain observational studies showing that, at least at z ∼> 1, active galaxies do not preferentially show merger signatures.

Ultrafast Silicon Photonics with Visible to Mid-Infrared Pumping of Silicon Nanocrystals.

Science.gov (United States)

Diroll, Benjamin T; Schramke, Katelyn S; Guo, Peijun; Kortshagen, Uwe R; Schaller, Richard D

2017-10-11

Dynamic optical control of infrared (IR) transparency and refractive index is achieved using boron-doped silicon nanocrystals excited with mid-IR optical pulses. Unlike previous silicon-based optical switches, large changes in transmittance are achieved without a fabricated structure by exploiting strong light coupling of the localized surface plasmon resonance (LSPR) produced from free holes of p-type silicon nanocrystals. The choice of optical excitation wavelength allows for selectivity between hole heating and carrier generation through intraband or interband photoexcitation, respectively. Mid-IR optical pumping heats the free holes of p-Si nanocrystals to effective temperatures greater than 3500 K. Increases of the hole effective mass at high effective hole temperatures lead to a subpicosecond change of the dielectric function, resulting in a redshift of the LSPR, modulating mid-IR transmission by as much as 27%, and increasing the index of refraction by more than 0.1 in the mid-IR. Low hole heat capacity dictates subpicosecond hole cooling, substantially faster than carrier recombination, and negligible heating of the Si lattice, permitting mid-IR optical switching at terahertz repetition frequencies. Further, the energetic distribution of holes at high effective temperatures partially reverses the Burstein-Moss effect, permitting the modulation of transmittance at telecommunications wavelengths. The results presented here show that doped silicon, particularly in micro- or nanostructures, is a promising dynamic metamaterial for ultrafast IR photonics.

Structure in continuously cored, deep drill holes at Yucca Mountain, Nevada, with notes on calcite occurrence

International Nuclear Information System (INIS)

Carr, W.J.

1992-12-01

A study of more than 22,000 feet of core from five deep drill holes at Yucca Mountain, Nevada, provided data on the attitude and vertical distribution of faults and fractures, the sense of fault displacement, and the occurrence of calcite. The study was done mainly to look for evidence of fault flattening at depth, but no consistent downward decrease in dip of faults was found, and no increase in strata rotation was evident with increasing depth. In the two drill holes located near prominent faults that dip toward the holes (USW G-3 and G-2), an apparent increase in the frequency of faults occurs below the tuffs and lavas of Calico Hills. Some of this increase occurs in brittle lavas and flow breccias in the lower part of the volcanic section. In the two holes presumed to be relatively removed from the influence of important faults at depth, the vertical distribution of faults is relatively uniform. Calcite occurs mainly in two general zones, voids in welded portions of the Paintbrush Tuff, and in a deeper zone, mostly below 3,500 feet. Calcite is least abundant in USW G-4, which may reflect the fewer faults and fractures encountered in that drill hole

Extended two-temperature model for ultrafast thermal response of band gap materials upon impulsive optical excitation

Energy Technology Data Exchange (ETDEWEB)

Shin, Taeho [Department of Chemistry, Massachusetts Institute of Technology, Cambridge, Massachusetts 02139-4307 (United States); Samsung Advanced Institute of Technology, Suwon 443-803 (Korea, Republic of); Teitelbaum, Samuel W.; Wolfson, Johanna; Nelson, Keith A., E-mail: kanelson@mit.edu [Department of Chemistry, Massachusetts Institute of Technology, Cambridge, Massachusetts 02139-4307 (United States); Kandyla, Maria [Department of Chemistry, Massachusetts Institute of Technology, Cambridge, Massachusetts 02139-4307 (United States); Theoretical and Physical Chemistry Institute, National Hellenic Research Foundation, Athens 116-35 (Greece)

2015-11-21

Thermal modeling and numerical simulations have been performed to describe the ultrafast thermal response of band gap materials upon optical excitation. A model was established by extending the conventional two-temperature model that is adequate for metals, but not for semiconductors. It considers the time- and space-dependent density of electrons photoexcited to the conduction band and accordingly allows a more accurate description of the transient thermal equilibration between the hot electrons and lattice. Ultrafast thermal behaviors of bismuth, as a model system, were demonstrated using the extended two-temperature model with a view to elucidating the thermal effects of excitation laser pulse fluence, electron diffusivity, electron-hole recombination kinetics, and electron-phonon interactions, focusing on high-density excitation.

A PSF-shape-based beamforming strategy for robust 2D motion estimation in ultrafast data

NARCIS (Netherlands)

Saris, Anne E.C.M.; Fekkes, Stein; Nillesen, Maartje; Hansen, Hendrik H.G.; de Korte, Chris L.

2018-01-01

This paper presents a framework for motion estimation in ultrafast ultrasound data. It describes a novel approach for determining the sampling grid for ultrafast data based on the system's point-spread-function (PSF). As a consequence, the cross-correlation functions (CCF) used in the speckle

Gaspe hole sets depth record

Energy Technology Data Exchange (ETDEWEB)

1970-03-09

The deepest diamond-cored hole in the Western Hemisphere, Gulf Sunnybank No. 1 on the Gaspe Peninsula of Quebec, has been completed at a depth of 11,600 ft. This is the deepest cored hole to be drilled anywhere in search of oil and gas production, and the deepest to be drilled using a wire-line core recovery technique. The well was completed in 183 days, and was cored continuously below the surface casing which was set and cemented at 1,004 ft. After underreaming a portion of the bottom of the hole, intermediate casing was set and cemented at 8,000 ft as a safety precaution against possible high oil or gas-fluid pressure. Actual coring time, after deducting time for underreaming and casing operations, was 152 days. Because of the cost of transporting a conventional oil-drilling rig to the E. location, the 89-ft mining rig was modified for the project. The contractor was Heath and Sherwood Drilling (Western) Ltd.

Nondestructive continuous physical property measurements of core samples recovered from hole B, Taiwan Chelungpu-Fault Drilling Project

Science.gov (United States)

Hirono, Tetsuro; Yeh, En-Chao; Lin, Weiren; Sone, Hiroki; Mishima, Toshiaki; Soh, Wonn; Hashimoto, Yoshitaka; Matsubayashi, Osamu; Aoike, Kan; Ito, Hisao; Kinoshita, Masataka; Murayama, Masafumi; Song, Sheng-Rong; Ma, Kuo-Fong; Hung, Jih-Hao; Wang, Chien-Ying; Tsai, Yi-Ben; Kondo, Tomomi; Nishimura, Masahiro; Moriya, Soichi; Tanaka, Tomoyuki; Fujiki, Toru; Maeda, Lena; Muraki, Hiroaki; Kuramoto, Toshikatsu; Sugiyama, Kazuhiro; Sugawara, Toshikatsu

2007-07-01

The Taiwan Chelungpu-Fault Drilling Project was undertaken in 2002 to investigate the faulting mechanism of the 1999 Mw 7.6 Taiwan Chi-Chi earthquake. Hole B penetrated the Chelungpu fault, and core samples were recovered from between 948.42- and 1352.60-m depth. Three major zones, designated FZB1136 (fault zone at 1136-m depth in hole B), FZB1194, and FZB1243, were recognized in the core samples as active fault zones within the Chelungpu fault. Nondestructive continuous physical property measurements, conducted on all core samples, revealed that the three major fault zones were characterized by low gamma ray attenuation (GRA) densities and high magnetic susceptibilities. Extensive fracturing and cracks within the fault zones and/or loss of atoms with high atomic number, but not a measurement artifact, might have caused the low GRA densities, whereas the high magnetic susceptibility values might have resulted from the formation of magnetic minerals from paramagnetic minerals by frictional heating. Minor fault zones were characterized by low GRA densities and no change in magnetic susceptibility, and the latter may indicate that these minor zones experienced relatively low frictional heating. Magnetic susceptibility in a fault zone may be key to the determination that frictional heating occurred during an earthquake on the fault.

Many-particle correlations in quasi-two-dimensional electron-hole systems

International Nuclear Information System (INIS)

Nikolaev, Valentin

2002-01-01

This thesis reports a theoretical investigation of many-particle correlation effects in semiconductor heterostructures containing quantum wells. Particular attention is paid towards quasi-particle pair correlations. Using the Green's function technique and the ladder approximation as a basis, the generalized mass action law, which describes the redistribution of particles between correlated and uncorrelated states in quasi-two-dimensional systems for different temperatures and total densities, is derived. The expression is valid beyond the low-density limit, which allows us to investigate the transition of the system from a dilute exciton gas to a dense electron-hole plasma. A generalized Levinson theorem, which takes k-space filling into account, is formulated. Screening in quasi-two-dimensional systems is analyzed rigorously. Firstly, the qualitatively new mechanism of static local screening by indirect excitons is studied using the simple Thomas-Fermi approximation. Then, a detailed many-body description suitable for a proper account of dynamic screening by a quasi-2D electron-hole plasma, and consistent with the previously derived mass action law, is provided. The generalized Lindhard approximation and excitonic plasmon-pole approximations are also derived. The theory is applied to single and double quantum wells. A self-consistent procedure is developed for numerical investigation of the ionization degree of an electron-hole plasma at different values of temperature/exciton Rydberg ratios. This procedure accounts for screening, k-space filling (exciton bleaching), and the formation of excitons. An abrupt jump in the value of the ionization degree that happens with an increase of the carrier density or temperature (Mott transition) is found in a certain density-temperature region. It has been found that the critical density of the Mott transition for indirect excitons may be much smaller than that for direct excitons. A suggestion has been made that some of the

Fourteenth International Conference on Ultrafast Phenomena

CERN Document Server

Kobayashi, Takayoshi; Kobayashi, Tetsuro; Nelson, Keith A; Silvestri, Sandro; Ultrafast Phenomena XIV

2005-01-01

Ultrafast Phenomena XIV presents the latest advances in ultrafast science, including ultrafast laser and measurement technology as well as studies of ultrafast phenomena. Pico-, femto-, and atosecond processes relevant in physics, chemistry, biology and engineering are presented. Ultrafast technology is now having a profound impact within a wide range of applications, among them imaging, material diagnostics, and transformation and high-speed optoelectronics. This book summarizes results presented at the 14th Ultrafast Phenomena Conference and reviews the state of the art in this important and rapidly advancing field.

Sixteenth International Conference on Ultrafast Phenomena

CERN Document Server

Corkum, Paul; Nelson, Keith A; Riedle, Eberhard; Schoenlein, Robert W; Ultrafast Phenomena XVI

2009-01-01

Ultrafast Phenomena XVI presents the latest advances in ultrafast science, including both ultrafast optical technology and the study of ultrafast phenomena. It covers picosecond, femtosecond and attosecond processes relevant to applications in physics, chemistry, biology, and engineering. Ultrafast technology has a profound impact in a wide range of applications, amongst them biomedical imaging, chemical dynamics, frequency standards, material processing, and ultrahigh speed communications. This book summarizes the results presented at the 16th International Conference on Ultrafast Phenomena and provides an up-to-date view of this important and rapidly advancing field.

Nearly suppressed photoluminescence blinking of small-sized, blue-green-orange-red emitting single CdSe-based core/gradient alloy shell/shell quantum dots: correlation between truncation time and photoluminescence quantum yield.

Science.gov (United States)

Roy, Debjit; Mandal, Saptarshi; De, Chayan K; Kumar, Kaushalendra; Mandal, Prasun K

2018-04-18

CdSe-based core/gradient alloy shell/shell semiconductor quantum dots (CGASS QDs) have been shown to be optically quite superior compared to core-shell QDs. However, very little is known about CGASS QDs at the single particle level. Photoluminescence blinking dynamics of four differently emitting (blue (λem = 510), green (λem = 532), orange (λem = 591), and red (λem = 619)) single CGASS QDs having average sizes 600 nm). In this manuscript, we report nearly suppressed PL blinking behaviour of CGASS QDs with average sizes correlation between the event durations and found that residual memory exists in both the ON- and OFF-event durations. Positively correlated successive ON-ON and OFF-OFF event durations and negatively correlated (anti-correlated) ON-OFF event durations perhaps suggest the involvement of more than one type of trapping process within the blinking framework. The timescale corresponding to the additional exponential term has been assigned to hole trapping for ON-event duration statistics. Similarly, for OFF-event duration statistics, this component suggests hole detrapping. We found that the average duration of the exponential process for the ON-event durations is an order of magnitude higher than that of the OFF-event durations. This indicates that the holes are trapped for a significantly long time. When electron trapping is followed by such a hole trapping, long ON-event durations result. We have observed long ON-event durations, as high as 50 s. The competing charge tunnelling model has been used to account for the observed blinking behaviour in these CGASS QDs. Quite interestingly, the PLQY of all of these differently emitting QDs (an ensemble level property) could be correlated with the truncation time (a property at the single particle level). A respective concomitant increase-decrease of ON-OFF event truncation times with increasing PLQY is also indicative of a varying degree of suppression of the Auger recombination processes in these four

Hole history, rotary hole DC-3

International Nuclear Information System (INIS)

1977-10-01

Purpose of hole DC-3 was to drill into the Umtanum basalt flow using both conventional rotary and core drilling methods. The borehole is to be utilized for geophysical logging, future hydrological testing, and the future installation of a borehole laboratory for long-term pressure, seismic, and moisture migration or accumulation recording in the Umtanum basalt flow in support of the Basalt Waste Isolation Program. Hole DC-3 is located east of the 200 West barricaded area on the Hanford reservation

The interpretation of geochemical logs from the oceanic basement: mineral modelling in Ocean Drilling Program (ODP) Hole 735B

International Nuclear Information System (INIS)

Harvey, P.K.; Lovell, M.A.; Bristow, J.F.

1991-01-01

Leg 118 of the Ocean Drilling Program was carried out in the vicinity of the Southwest Indian Ridge. Of the boreholes drilled, by far the most important and scientifically spectacular is Hole 735B which was located on a shallow platform adjacent to the Atlantis II Transform. This hole penetrates some 500 m of gabbroic rocks representing Layer 3 of the oceanic crust. The recovered gabbros show considerable variation both in mineralogy and in the degree of deformation. Core recovery averages 87% and there is excellent control and correlation between the core and the wide range of logs obtained. Mineralogy logs are derived and presented using both core sample data and downhole geochemical logs for Hole 735B. The problems of transforming these data for the particular mineralogy encountered are discussed. (Author)

Coulomb holes and correlation potentials in the helium atom

International Nuclear Information System (INIS)

Slamet, M.; Sahni, V.

1995-01-01

Thus, the asymptotic structure of the exchange-correlation potential W xc (r) of the work formalism is that of W x (r) which is (-1/r). We also detemine via the Kinoshita wave function the correlation potential μ c (r) of Kohn-Sham theory, which differs from W c (r) in that it also incorporates the effects of the correlation contribution to the kinetic energy. Consequently, it is less attractive than W c (r), but also has zero slope at the nucleus. However, as is known, the potential μ c (r) is nonmonotonic, since it goes positive within the atom, then becomes negative in the classically forbidden region, finally vanishing asymptotically as a negative function. Since the exchange potentials of the work formalism and Kohn-Sham theory are the same for this atom, and because W c (r) is strictly representative of Coulomb correlations, we attribute the nonmonotonicity and positiveness of the Kohn-Sham potential μ c (r) to the correlation kinetic energy. This conclusion is consistent with the result that the difference between the correlation energies determined within the work formalism from the dynamic Coulomb hole and Kohn-Sham theory is equal to the correlation contribution to the kinetic energy

Ultrafast time measurements by time-correlated single photon counting coupled with superconducting single photon detector

Energy Technology Data Exchange (ETDEWEB)

Shcheslavskiy, V., E-mail: vis@becker-hickl.de; Becker, W. [Becker & Hickl GmbH, Nahmitzer Damm 30, 12277 Berlin (Germany); Morozov, P.; Divochiy, A. [Scontel, Rossolimo St., 5/22-1, Moscow 119021 (Russian Federation); Vakhtomin, Yu. [Scontel, Rossolimo St., 5/22-1, Moscow 119021 (Russian Federation); Moscow State Pedagogical University, 1/1 M. Pirogovskaya St., Moscow 119991 (Russian Federation); Smirnov, K. [Scontel, Rossolimo St., 5/22-1, Moscow 119021 (Russian Federation); Moscow State Pedagogical University, 1/1 M. Pirogovskaya St., Moscow 119991 (Russian Federation); National Research University Higher School of Economics, 20 Myasnitskaya St., Moscow 101000 (Russian Federation)

2016-05-15

Time resolution is one of the main characteristics of the single photon detectors besides quantum efficiency and dark count rate. We demonstrate here an ultrafast time-correlated single photon counting (TCSPC) setup consisting of a newly developed single photon counting board SPC-150NX and a superconducting NbN single photon detector with a sensitive area of 7 × 7 μm. The combination delivers a record instrument response function with a full width at half maximum of 17.8 ps and system quantum efficiency ∼15% at wavelength of 1560 nm. A calculation of the root mean square value of the timing jitter for channels with counts more than 1% of the peak value yielded about 7.6 ps. The setup has also good timing stability of the detector–TCSPC board.

Electron-mediated relaxation following ultrafast pumping of strongly correlated materials: model evidence of a correlation-tuned crossover between thermal and nonthermal states.

Science.gov (United States)

Moritz, B; Kemper, A F; Sentef, M; Devereaux, T P; Freericks, J K

2013-08-16

We examine electron-electron mediated relaxation following ultrafast electric field pump excitation of the fermionic degrees of freedom in the Falicov-Kimball model for correlated electrons. The results reveal a dichotomy in the temporal evolution of the system as one tunes through the Mott metal-to-insulator transition: in the metallic regime relaxation can be characterized by evolution toward a steady state well described by Fermi-Dirac statistics with an increased effective temperature; however, in the insulating regime this quasithermal paradigm breaks down with relaxation toward a nonthermal state with a complicated electronic distribution as a function of momentum. We characterize the behavior by studying changes in the energy, photoemission response, and electronic distribution as functions of time. This relaxation may be observable qualitatively on short enough time scales that the electrons behave like an isolated system not in contact with additional degrees of freedom which would act as a thermal bath, especially when using strong driving fields and studying materials whose physics may manifest the effects of correlations.

Electron–hole two-stream instability in a quantum semiconductor plasma with exchange-correlation effects

International Nuclear Information System (INIS)

Zeba, I.; Yahia, M.E.; Shukla, P.K.; Moslem, W.M.

2012-01-01

The electron–hole two-stream instability in a quantum semiconductor plasma has been studied including electrons and holes quantum recoil effects, exchange-correlation potentials, and degenerate pressures of the plasma species. Typical values of GaAs and GaSb semiconductors are used to estimate the growth rate of the two-stream instability. The effects of electron– and hole–phonon collision, quantum recoil effects, the streaming velocities, and the corresponding threshold on the growth rate are investigated numerically. Considering the phonon susceptibility allows the acoustic mode to exist and the collisional instability arises in combination with drift of the holes. -- Highlights: ► Electron–hole two stream instability in quantum plasmas is presented. ► Typical values of GaAs and GaSb semiconductors are used to estimate the growth rate. ► The streaming velocities and the corresponding threshold on the growth rate are investigated numerically.

A comparative theoretical study on core-hole excitation spectra of azafullerene and its derivatives

Energy Technology Data Exchange (ETDEWEB)

Deng, Yunfeng [Guizhou Provincial Key Laboratory of Computational Nano-material Science, Guizhou Normal College, Guiyang 550018 (China); Department of Physics, Guizhou University, Guiyang 550025 (China); Gao, Bin, E-mail: bin.gao@uit.no [Guizhou Provincial Key Laboratory of Computational Nano-material Science, Guizhou Normal College, Guiyang 550018 (China); Centre for Theoretical and Computational Chemistry (CTCC), Department of Chemistry, University of Tromsø—The Arctic University of Norway, N-9037 Tromsø (Norway); Deng, Mingsen, E-mail: deng@gznc.edu.cn [Guizhou Provincial Key Laboratory of Computational Nano-material Science, Guizhou Normal College, Guiyang 550018 (China); Luo, Yi [Guizhou Provincial Key Laboratory of Computational Nano-material Science, Guizhou Normal College, Guiyang 550018 (China); Department of Theoretical Chemistry, School of Biotechnology, Royal Institute of Technology, SE-10691 Stockholm (Sweden)

2014-03-28

The core-hole excitation spectra—near-edge x-ray absorption spectroscopy (NEXAFS), x-ray emission spectroscopy (XES), and x-ray photoelectron spectroscopy (XPS) shake-up satellites have been simulated at the level of density functional theory for the azafullerene C{sub 59}N and its derivatives (C{sub 59}N){sup +}, C{sub 59}HN, (C{sub 59}N){sub 2}, and C{sub 59}N–C{sub 60}, in which the XPS shake-up satellites were simulated using our developed equivalent core hole Kohn-Sham (ECH-KS) density functional theory approach [B. Gao, Z. Wu, and Y. Luo, J. Chem. Phys. 128, 234704 (2008)] which aims for the study of XPS shake-up satellites of large-scale molecules. Our calculated spectra are generally in good agreement with available experimental results that validates the use of the ECH-KS method in the present work. The nitrogen K-edge NEXAFS, XES, and XPS shake-up satellites spectra in general can be used as fingerprints to distinguish the azafullerene C{sub 59}N and its different derivatives. Meanwhile, different carbon K-edge spectra could also provide detailed information of (local) electronic structures of different molecules. In particular, a peak (at around 284.5 eV) in the carbon K-edge NEXAFS spectrum of the heterodimer C{sub 59}N–C{sub 60} is confirmed to be related to the electron transfer from the C{sub 59}N part to the C{sub 60} part in this charge-transfer complex.

XFEL resonant photo-pumping of dense plasmas and dynamic evolution of autoionizing core hole states

OpenAIRE

Rosmej, F. B.; Moinard, A.; Renner, O.; Galtier, E.; Lee, J. J.; Nagler, B.; Heimann, P. A.; Schlotter, W.; Turner, J. J.; Lee, R. W.; Makita, M.; Riley, D.; Seely, J.

2016-01-01

Similarly to the case of LIF (Laser-Induced Fluorescence), an equally revolutionary impact to science is expected from resonant X-ray photo-pumping. It will particularly contribute to a progress in high energy density science: pumped core hole states create X-ray transitions that can escape dense matter on a 10 fs-time scale without essential photoabsorption, thus providing a unique possibility to study matter under extreme conditions. In the first proof of principle experiment at the X-ray F...

Silicon as a virtual plasmonic material: Acquisition of its transient optical constants and the ultrafast surface plasmon-polariton excitation

Energy Technology Data Exchange (ETDEWEB)

Danilov, P. A.; Ionin, A. A.; Kudryashov, S. I., E-mail: sikudr@sci.lebedev.ru; Makarov, S. V.; Rudenko, A. A. [Lebedev Physical Institute (Russian Federation); Saltuganov, P. N. [Moscow Institute of Physics and Technology (State University) (Russian Federation); Seleznev, L. V.; Yurovskikh, V. I.; Zayarny, D. A. [Lebedev Physical Institute (Russian Federation); Apostolova, T. [Bulgarian Academy of Sciences, Institute for Nuclear Research and Nuclear Energetics (Bulgaria)

2015-06-15

Ultrafast intense photoexcitation of a silicon surface is complementarily studied experimentally and theoretically, with its prompt optical dielectric function obtained by means of time-resolved optical reflection microscopy and the underlying electron-hole plasma dynamics modeled numerically, using a quantum kinetic approach. The corresponding transient surface plasmon-polariton (SPP) dispersion curves of the photo-excited material were simulated as a function of the electron-hole plasma density, using the derived optical dielectric function model, and directly mapped at several laser photon energies, measuring spatial periods of the corresponding SPP-mediated surface relief nanogratings. The unusual spectral dynamics of the surface plasmon resonance, initially increasing with the increase in the electron-hole plasma density but damped at high interband absorption losses induced by the high-density electron-hole plasma through instantaneous bandgap renormalization, was envisioned through the multi-color mapping.

Search for gravitational waves on short duration in TAMA300 data: stellar core collapse and black hole

International Nuclear Information System (INIS)

Honda, R; Kanda, N; Akutsu, T; Ando, M; Tsunesada, Y

2008-01-01

We present in the results of TAMA300 data analysis for short duration gravitational waves. The excess power filter, alternative linear filter (ALF) and TF(time-frequency) clustering methods have been employed for burst gravitational waves from stellar-core collapse, and matched filtering method used for the ringdown gravitational waves from black hole quasi-normal oscillations. The observational range of TAMA for the burst gravitational waves is roughly ∼ 1 kpc, and the range for black hole ringdown covers most of our galaxy. We have been developed new method 'time-frequency (TF) clustering' to find the burst waves. This is a TF clustering method on spectrogram (sonogram). Using this method, we can efficiently identify some predicted gravitational wave forms and can exclude typical unstable spike like noises

Ultrafast magnetic vortex core switching driven by the topological inverse Faraday effect.

Science.gov (United States)

Taguchi, Katsuhisa; Ohe, Jun-ichiro; Tatara, Gen

2012-09-21

We present a theoretical discovery of an unconventional mechanism of inverse Faraday effect which acts selectively on topological magnetic structures. The effect, topological inverse Faraday effect, is induced by the spin Berry's phase of the magnetic structure when a circularly polarized light is applied. Thus a spin-orbit interaction is not necessary unlike that in the conventional inverse Faraday effect. We demonstrate by numerical simulation that topological inverse Faraday effect realizes ultrafast switching of a magnetic vortex within a switching time of 150 ps without magnetic field.

Impact of local order and stoichiometry on the ultrafast magnetization dynamics of Heusler compounds

International Nuclear Information System (INIS)

Steil, Daniel; Schmitt, Oliver; Fetzer, Roman; Aeschlimann, Martin; Cinchetti, Mirko; Kubota, Takahide; Naganuma, Hiroshi; Oogane, Mikihiko; Ando, Yasuo; Rodan, Steven; Blum, Christian G F; Wurmehl, Sabine; Balke, Benjamin

2015-01-01

Nowadays, a wealth of information on ultrafast magnetization dynamics of thin ferromagnetic films exists in the literature. Information is, however, scarce on bulk single crystals, which may be especially important for the case of multi-sublattice systems. In Heusler compounds, representing prominent examples for such multi-sublattice systems, off-stoichiometry and degree of order can significantly change the magnetic properties of thin films, while bulk single crystals may be generally produced with a much more well-defined stoichiometry and a higher degree of ordering. A careful characterization of the local structure of thin films versus bulk single crystals combined with ultrafast demagnetization studies can, thus, help to understand the impact of stoichiometry and order on ultrafast spin dynamics.Here, we present a comparative study of the structural ordering and magnetization dynamics for thin films and bulk single crystals of the family of Heusler alloys with composition Co 2 Fe 1 − x Mn x Si. The local ordering is studied by 59 Co nuclear magnetic resonance (NMR) spectroscopy, while the time-resolved magneto-optical Kerr effect gives access to the ultrafast magnetization dynamics. In the NMR studies we find significant differences between bulk single crystals and thin films, both regarding local ordering and stoichiometry. The ultrafast magnetization dynamics, on the other hand, turns out to be mostly unaffected by the observed structural differences, especially on the time scale of some hundreds of femtoseconds. These results confirm hole-mediated spin-flip processes as the main mechanism for ultrafast demagnetization and the robustness of this demagnetization channel against defect states in the minority band gap as well as against the energetic position of the band gap with respect to the Fermi energy. The very small differences observed in the magnetization dynamics on the picosecond time-scale, on the other hand, can be explained by considering the

Ultrafast MR Imaging in Pediatric Neuroradiology

International Nuclear Information System (INIS)

Singh, R.K.; Smith, J.T.; Wilkinson, I.D.; Griffiths, P.D.

2003-01-01

Purpose: To compare the diagnostic information obtained from ultrafast MR imaging with standard MR imaging techniques in pediatric neuroradiology. The goal was to judge whether ultrafast methods can be used to replace standard methods and reduce the need for sedation or general anesthesia as a result of the considerably shorter scan times. Material and Methods: Our prospective study involved 125 patients. Routine clinical imaging was performed along with two ultrafast methods. Single shot fast spin echo (SSFSE) was used to give T2-weighted images and an echo planar imaging (EPI) sequence to provide a T1-weighted images. The ultrafast images were presented to an experienced neuro radiologist who was also given the information present on the initial referral card. These reports based on the ultrafast images were then compared with the formal radiologic report made solely on the basis of the standard imaging. Results: The overall sensitivity and specificity for ultrafast imaging when compared to the reference standard were 78% and 98% with positive and negative predictive values of 98% and 76%. Pathologies characterized by small areas of subtle T2 prolongation were difficult or impossible to see on the ultrafast images but otherwise they provided reliable information. Conclusions: This paper demonstrates that ultrafast MR imaging can diagnose many pediatric intracranial abnormalities as well as standard methods. Anatomic resolution limits its capacity to define subtle developmental anomalies and contrast resolution limitations of the ultrafast methods reduce the detection of pathology characterized by subtle T2 prolongation

Spectral hole-burning and carrier-heating dynamics in quantum-dot amplifiers: Comparison with bulk amplifiers

DEFF Research Database (Denmark)

Borri, P.; Langbein, W.; Hvam, Jørn Märcher

2001-01-01

The ultrafast gain dynamics in an electrically pumped InAs/InGaAs/GaAs quantum-dot amplifier are measured at room temperature with femtosecond resolution, and compared with results on an InGaAsP bulk amplifier. The role of spectral hole burning and carrier heating in the recovery of the gain...

Ultra-Fast Outflows in Radio-Loud AGN: New Constraints on Jet-Disk Connection

Science.gov (United States)

Sambruna, Rita

There is strong observational and theoretical evidence that outflows/jets are coupled to accretion disks in black hole accreting systems, from Galactic to extragalactic sizes. While in radio-quiet AGN there is ample evidence for the presence of Ultra-Fast Outflows (UFOs) from the presence of blue-shifted absorption features in their 4-10~keV spectra, sub-relativistic winds are expected on theoretical basis in radio-loud AGN but have not been observed until now. Our recent Suzaku observations of 5 bright Broad- Line Radio Galaxies (BLRGs, the radio-loud counterparts of Seyferts) has started to change this picture. We found strong evidence for UFOs in 3 out of 5 BLRGs, with ionization parameters, column densities, and velocities of the absorber similar to Seyferts. Moreover, the outflows in BLRGs are likely to be energetically very significant: from the Suzaku data of the three sources, outflow masses similar to the accretion masses and kinetic energies of the wind similar to the X-ray luminosity and radio power of the jet are inferred. Clearly, UFOs in radio-loud AGN represent a new key ingredient to understand their central engines and in particular, the jet-disk linkage. Our discovery of UFOs in a handful of BLRGs raises the questions of how common disk winds are in radio-loud AGN, what the absorber physical and dynamical characteristics are, and what is the outflow role in broader picture of galaxy-black hole connection for radio sources, i.e., for large-scale feedback models. To address these and other issues, we propose to use archival XMM-Newton and Suzaku spectra to search for Ultra-Fast Outflows in a large number of radio sources. Over a period of two years, we will conduct a systematic, uniform analysis of the archival X-ray data, building on our extensive experience with a similar previous project for Seyferts, and using robust analysis and statistical methodologies. As an important side product, we will also obtain accurate, self- consistent measurements

Hole energy and momentum distributions in valence bands

International Nuclear Information System (INIS)

Laan, G. van der.

1982-01-01

In order to understand the electrical and magnetic properties of solids, the knowledge of the density of states and the dispersion relation of the valence bands is indispensable. This thesis offers some alternative methods to obtain information about the nature of the valence band. Part A deals with the energy distribution of the photoelectrons. A simple model, which explains the core hole satellite structure in compounds with large correlation effects between the valence band holes and the created photo-hole, is outlined. CuCl, CuX 2 (X = F Cl and Br) are studied, by photoemission and Auger electron spectroscopies in determining the valence band properties. Part B deals with the simultaneous measurement of the energy and the wave vector of the emitted electrons. A practical example is given for the determination of the dispersion relation in copper. The measurements of a surface resonance band and the distribution of the secondary electrons are also reported. (Auth.)

Ultrafast photoelectron spectroscopy of small molecule organic films

Science.gov (United States)

Read, Kendall Laine

As research in the field of ultrafast optics has produced shorter and shorter pulses, at an ever-widening range of frequencies, ultrafast spectroscopy has grown correspondingly. In particular, ultrafast photoelectron spectroscopy allows direct observation of electrons in transient or excited states, regardless of the eventual relaxation mechanisms. High-harmonic conversion of 800nm, femtosecond, Ti:sapphire laser pulses allows excite/probe spectroscopy down into atomic core level states. To this end, an ultrafast, X-UV photoelectron spectroscopic system is described, including design considerations for the high-harmonic generation line, the time of flight detector, and the subsequent data collection electronics. Using a similar experimental setup, I have performed several ultrafast, photoelectron excited state decay studies at the IBM, T. J. Watson Research Center. All of the observed materials were electroluminescent thin film organics, which have applications as the emitter layer in organic light emitting devices. The specific materials discussed are: Alq, BAlq, DPVBi, and Alq doped with DCM or DMQA. Alq:DCM is also known to lase at low photoexcitation thresholds. A detailed understanding of the involved relaxation mechanisms is beneficial to both applications. Using 3.14 eV excite, and 26.7 eV probe, 90 fs laser pulses, we have observed the lowest unoccupied molecular orbital (LUMO) decay rate over the first 200 picoseconds. During this time, diffusion is insignificant, and all dynamics occur in the absence of electron transport. With excitation intensities in the range of 100μJ/cm2, we have modeled the Alq, BAlq, and DPVBi decays via bimolecular singlet-singlet annihilation. At similar excitations, we have modeled the Alq:DCM decay via Förster transfer, stimulated emission, and excimeric formation. Furthermore, the Alq:DCM occupied to unoccupied molecular orbital energy gap was seen to shrink as a function of excite-to-probe delay, in accordance with the

Black Holes and Galactic Density Cusps I Radial Orbit Cusps and Bulges

CERN Document Server

Henriksen, Richard N; Macmillan, Joseph D

2011-01-01

Aims. In this paper we study density cusps made from radial orbits that may contain central black holes. The actual co-eval self-similar growth would not distinguish between the central object and the surroundings. Methods. To study the environment of an existing black hole we seek distribution functions that may contain a black hole and that retain at least a memory of self-similarity. We refer to the environment in brief as the 'bulge' or sometimes the 'halo'. This depends on whether the black hole is a true singularity dominating its halo or rather a core mass concentration that dominates a larger bulge. The hierarchy might extend to include galactic bulge and halo. Results.We find simple descriptions of simulated collisionless matter in the process of examining the presence of central masses. The Fridmann & Polyachenko distribution function describes co-eval growth of a bulge and black hole that might explain the observed mass correlation. Conclusions. We derive our results from first principles assum...

Borehole geophysical measurements for Hole UE25a-3, Nevada Test Site, Nuclear Waste Isolation Program

International Nuclear Information System (INIS)

Daniels, J.J.; Scott, J.H.

1980-01-01

Borehole geophysical measurements made in drill hole UE25a-3 with a US Geological Survey research well-logging truck are presented in this paper. The purpose of these logging measurements is to provide in-situ physical properties information that is not commercially available on drill hole UE25a-3. Well logs are presented in this paper for dual-detector density, normal resistivity, gamma-ray, neutron-neutron, induced polarization, and magnetic susceptibility measurements. These data are analyzed correlations with the core lithology. Hole-to-surface measurements made from drill hole UE25a-3 indicate the presence of two resistive bodies at depth. The deeper resistive anomaly may be related to a granitic intrusion

Evidence for ultra-fast outflows in radio-quiet AGNs: III - location and energetics

OpenAIRE

Tombesi, F.; Cappi, M.; Reeves, J. N.; Braito, V.

2012-01-01

Using the results of a previous X-ray photo-ionization modelling of blue-shifted Fe K absorption lines on a sample of 42 local radio-quiet AGNs observed with XMM-Newton, in this letter we estimate the location and energetics of the associated ultra-fast outflows (UFOs). Due to significant uncertainties, we are essentially able to place only lower/upper limits. On average, their location is in the interval ~0.0003-0.03pc (~10^2-10^4 r_s) from the central black hole, consistent with what is exp...

Photon-trapping micro/nanostructures for high linearity in ultra-fast photodiodes

Science.gov (United States)

Cansizoglu, Hilal; Gao, Yang; Perez, Cesar Bartolo; Ghandiparsi, Soroush; Ponizovskaya Devine, Ekaterina; Cansizoglu, Mehmet F.; Yamada, Toshishige; Elrefaie, Aly F.; Wang, Shih-Yuan; Islam, M. Saif

2017-08-01

Photodetectors (PDs) in datacom and computer networks where the link length is up to 300 m, need to handle higher than typical input power used in other communication links. Also, to reduce power consumption due to equalization at high speed (>25Gb/s), the datacom links will use PAM-4 signaling instead of NRZ with stringent receiver linearity requirements. Si PDs with photon-trapping micro/nanostructures are shown to have high linearity in output current verses input optical power. Though there is less silicon material due to the holes, the micro-/nanostructured holes collectively reradiate the light to an in-plane direction of the PD surface and can avoid current crowding in the PD. Consequently, the photocurrent per unit volume remains at a low level contributing to high linearity in the photocurrent. We present the effect of design and lattice patterns of micro/nanostructures on the linearity of ultra-fast silicon PDs designed for high speed multi gigabit data networks.

Ultrafast Graphene Photonics and Optoelectronics

Science.gov (United States)

2017-04-14

AFRL-AFOSR-JP-TR-2017-0032 Ultrafast Graphene Photonics and Optoelectronics Kuang-Hsiung Wu National Chiao Tung University Final Report 04/14/2017...DATES COVERED (From - To) 18 Apr 2013 to 17 Apr 2016 4. TITLE AND SUBTITLE Ultrafast Graphene Photonics and Optoelectronics 5a.  CONTRACT NUMBER 5b...Prescribed by ANSI Std. Z39.18 Final Report for AOARD Grant FA2386-13-1-4022 “Ultrafast Graphene Photonics and Optoelectronics” Date May 23th, 2016

Ultrafast Science Opportunities with Electron Microscopy

Energy Technology Data Exchange (ETDEWEB)

DURR, HERMANN; Wang, X.J., ed.

2016-04-28

X-rays and electrons are two of the most fundamental probes of matter. When the Linac Coherent Light Source (LCLS), the world’s first x-ray free electron laser, began operation in 2009, it transformed ultrafast science with the ability to generate laser-like x-ray pulses from the manipulation of relativistic electron beams. This document describes a similar future transformation. In Transmission Electron Microscopy, ultrafast relativistic (MeV energy) electron pulses can achieve unsurpassed spatial and temporal resolution. Ultrafast temporal resolution will be the next frontier in electron microscopy and can ideally complement ultrafast x-ray science done with free electron lasers. This document describes the Grand Challenge science opportunities in chemistry, material science, physics and biology that arise from an MeV ultrafast electron diffraction & microscopy facility, especially when coupled with linac-based intense THz and X-ray pump capabilities.

Ultrafast Dephasing and Incoherent Light Photon Echoes in Organic Amorphous Systems

Science.gov (United States)

Yano, Ryuzi; Matsumoto, Yoshinori; Tani, Toshiro; Nakatsuka, Hiroki

1989-10-01

Incoherent light photon echoes were observed in organic amorphous systems (cresyl violet in polyvinyl alcohol and 1,4-dihydroxyanthraquinone in polymethacrylic acid) by using temporally-incoherent nanosecond laser pulses. It was found that an echo decay curve of an organic amorphous system is composed of a sharp peak which decays very rapidly and a slowly decaying wing at the tail. We show that the persistent hole burning (PHB) spectra were reproduced by the Fourier-cosine transforms of the echo decay curves. We claim that in general, we must take into account the multi-level feature of the system in order to explain ultrafast dephasing at very low temperatures.

Testing ultrafast mode-locking at microhertz relative optical linewidth.

Science.gov (United States)

Martin, Michael J; Foreman, Seth M; Schibli, T R; Ye, Jun

2009-01-19

We report new limits on the phase coherence of the ultrafast mode-locking process in an octave-spanning Ti:sapphire comb.We find that the mode-locking mechanism correlates optical phase across a full optical octave with less than 2.5 microHZ relative linewidth. This result is at least two orders of magnitude below recent predictions for quantum-limited individual comb-mode linewidths, verifying that the mode-locking mechanism strongly correlates quantum noise across the comb spectrum.

Testing ultrafast mode-locking at microhertz relative optical linewidth

OpenAIRE

Martin, Michael J.; Foreman, Seth M.; Schibli, T. R.; Ye, Jun

2008-01-01

We report new limits on the phase coherence of the ultrafast mode-locking process in an octave-spanning Ti:sapphire comb. We find that the mode-locking mechanism correlates optical phase across a full optical octave with less than 2.5 micro Hz relative linewidth. This result is at least two orders of magnitude below recent predictions for quantum-limited individual comb-mode linewidths, verifying that the mode-locking mechanism strongly correlates quantum noise across the comb spectrum.

Black holes new horizons

CERN Document Server

Hayward, Sean Alan

2013-01-01

Black holes, once just fascinating theoretical predictions of how gravity warps space-time according to Einstein's theory, are now generally accepted as astrophysical realities, formed by post-supernova collapse, or as supermassive black holes mysteriously found at the cores of most galaxies, powering active galactic nuclei, the most powerful objects in the universe. Theoretical understanding has progressed in recent decades with a wider realization that local concepts should characterize black holes, rather than the global concepts found in textbooks. In particular, notions such as trapping h

Star clusters containing massive, central black holes: evolution calculations

International Nuclear Information System (INIS)

Marchant, A.B.

1980-01-01

This dissertation presents a detailed, two-dimensional simulations of star cluster evolution. A Monte-Carlo method is adapted to simulate the development with time of isolated star clusters. Clusters which evolve on relaxation timescales with and without central black holes are treated. The method is flexible and rugged, rather than highly accurate. It treats the boundary conditions of stellar evaporation and tidal disruption by a central black hole in a precise, stochastic fashion. Dynamical cloning and renormalization and the use of a time-step adjustment algorithm enhance the feasibility of the method which simulates systems with wide ranges of intrinsic length and time scales. First, the method is applied to follow the development and core collapse of an initial Plummer-model cluster without a central black hole. Agreement of these results for early times with the results of previous authors serves as a verification of this method. Three calculations of cluster re-expansion, each beginning with the insertion of a black hole at the center of a highly collapsed cluster core is presented. Each case is characterized by a different value of initial black hole mass or black hole accretion efficiency for the consumption of debris from disrupted stars. It is found that for the special cases examined here substantial, but not catastrophic, growth of the central black hole may accompany core re-expansion. Also, the observability of the evolutionary phases associated with core collapse and re-expansion, constraints on x-ray sources which could be associated with growing black holes, and the observable signature of the cusp of stars surrounding a central black hole are discussed

Geochemistry of core samples of the Tiva Canyon Tuff from drill hole UE-25 NRG number-sign 3, Yucca Mountain, Nevada

International Nuclear Information System (INIS)

Peterman, Z.E.; Futa, K.

1996-01-01

The Tiva Canyon Tuff of Miocene age is composed of crystal-poor, high-silica rhyolite overlain by a crystal-rich zone that is gradational in composition from high-silica rhyolite to quartz latite. Each of these zones is divided into subzones that have distinctive physical, mineralogical, and geochemical features.Accurate identification of these subzones and their contacts is essential for detailed mapping and correlation both at the surface and in the subsurface in drill holes and in the exploratory studies facility (ESF). This report presents analyses of potassium (K), calcium (Ca), titanium (Ti), rubidium (Rb), strontium (Sr), yttrium (Y), zirconium (Zr), niobium (Nb), barium (Ba), lanthanum (La), and cerium (Ce) in core samples of the Tiva Canyon Tuff from drill hole UE-25 NRG number-sign 3. The concentrations of most of these elements are remarkably constant throughout the high-silica rhyolite, but at its upper contact with the crystal-rich zone, Ti, Zr, Ba, Ca, Sr, La, Ce, and K begin to increase progressively through the crystal-rich zone. In contrast, Rb and Nb decrease, and Y remains essentially constant. Initial 87 Sr/ 86 Sr ratios are relatively uniform in the high-silica rhyolite with a mean value of 0.7117, whereas initial 87 Sr/ 86 Sr ratios decrease upward in the quartz latite to values as low as 0.7090

Observation of plasma hole in a rotating plasma

International Nuclear Information System (INIS)

Nagaoka, Kenichi; Ishihara, Tatsuzo; Okamoto, Atsushi; Yoshimura, Shinji; Tanaka, Masayoshi Y.

2001-01-01

Plasma hole, a cylindrical density cavity, formed in a rotating plasma has been investigated experimentally. The plasma hole is characterized by large aspect ratio (length/radius ≥ 30), steep boundary layer between the hole and the ambient plasma (10 ion Larmor radius), and extremely high positive potential (130 V). The flow velocity field associated with plasma hole structure has been measured, and is found to have interesting features: (1) plasma rotates in azimuthal direction at a maximum velocity of order of ion sound speed, (2) plasma flows radially inward across the magnetic field line, (3) there present an axial flow reversal between core and peripheral region. It is found that the flow pattern of the plasma hole is very similar to the that of well-developed typhoon with core. (author)

X-ray absorption near-edge structure in alpha-quartz and stishovite: Ab initio calculation with core - hole interaction

International Nuclear Information System (INIS)

Mo, Shang-Di; Ching, W. Y.

2001-01-01

Ab initio calculation of the XANSE/ELNES spectra for α quartz and stishovite were carried out using a large-supercell approach that includes the electron - core - hole interaction. Excellent agreements with experimental spectra were obtained for Si - K, Si - L 2,3 , and O - K edges. The usual interpretation using orbital-resolved local density of states in the conduction band is unsatisfactory. [copyright] 2001 American Institute of Physics

Left ventricular ejection fraction and volumes as measured by 3D echocardiography and ultrafast computed tomography

International Nuclear Information System (INIS)

Vieira, Marcelo Luiz Campos; Nomura, Cesar H.; Tranchesi Junior, Bernardino; Oliveira, Wercules A. de; Naccarato, Gustavo; Serpa, Bruna S.; Passos, Rodrigo B.D.; Funari, Marcelo B. G.; Fischer, Claudio H.; Morhy, Samira S.

2009-01-01

Background: Real-time three-dimensional echocardiography (RT-3D-Echo) and ultrafast computed tomography (CT) are two novel methods for the analysis of LV ejection fraction and volumes. Objective: To compare LVEF and volume measurements as obtained using RT-3D-Echo and ultrafast CT. Methods: Thirty nine consecutive patients (27 men, mean age of 57+- 12 years) were studied using RT-3D-Echo and 64-slice ultrafast CT. LVEF and LV volumes were analyzed. Statistical analysis: coefficient of correlation (r: Pearson), Bland-Altman analysis, linear regression analysis, 95% CI, p 5 .58)%; end-diastolic volume ranged from 49.6 to 178.2 (87+-27.8) ml; end-systolic volume ranged from 11.4 to 78 (33.1+-13.6) ml. CT scan measurements: LVEF ranged from 53 to 86% (67.8+-7.78); end-diastolic volume ranged from 51 to 186 (106.5+-30.3) ml; end-systolic volume ranged from 7 to 72 (35.5+-13.4)ml. Correlations between RT-3D-Echo and CT were: LVEF (r: 0.7888, p<0.0001, 95% CI 0.6301 to 0.8843); end-diastolic volume (r: 0.7695, p<0.0001, 95% CI 0.5995 to 0.8730); end-systolic volume (r: 0.8119, p<0.0001, 95% CI 0.6673 to 0.8975). Conclusion: Good correlation between LVEF and ventricular volume parameters as measured by RT-3D-Echo and 64-slice ultrafast CT was found in the present case series. (author)

Interfacial charge separation and recombination in InP and quasi-type II InP/CdS core/shell quantum dot-molecular acceptor complexes.

Science.gov (United States)

Wu, Kaifeng; Song, Nianhui; Liu, Zheng; Zhu, Haiming; Rodríguez-Córdoba, William; Lian, Tianquan

2013-08-15

Recent studies of group II-VI colloidal semiconductor heterostuctures, such as CdSe/CdS core/shell quantum dots (QDs) or dot-in-rod nanorods, show that type II and quasi-type II band alignment can facilitate electron transfer and slow down charge recombination in QD-molecular electron acceptor complexes. To explore the general applicability of this wave function engineering approach for controlling charge transfer properties, we investigate exciton relaxation and dissociation dynamics in InP (a group III-V semiconductor) and InP/CdS core/shell (a heterostructure beween group III-V and II-VI semiconductors) QDs by transient absorption spectroscopy. We show that InP/CdS QDs exhibit a quasi-type II band alignment with the 1S electron delocalized throughout the core and shell and the 1S hole confined in the InP core. In InP-methylviologen (MV(2+)) complexes, excitons in the QD can be dissociated by ultrafast electron transfer to MV(2+) from the 1S electron level (with an average time constant of 11.4 ps) as well as 1P and higher electron levels (with a time constant of 0.39 ps), which is followed by charge recombination to regenerate the complex in its ground state (with an average time constant of 47.1 ns). In comparison, InP/CdS-MV(2+) complexes show similar ultrafast charge separation and 5-fold slower charge recombination rates, consistent with the quasi-type II band alignment in these heterostructures. This result demonstrates that wave function engineering in nanoheterostructures of group III-V and II-VI semiconductors provides a promising approach for optimizing their light harvesting and charge separation for solar energy conversion applications.

Proton-hole and core-excited states in the semi-magic nucleus {sup 131}In{sub 82}

Energy Technology Data Exchange (ETDEWEB)

Taprogge, J. [Instituto de Estructura de la Materia, CSIC, Madrid (Spain); Universidad Autonoma de Madrid, Departamento de Fisica Teorica, Madrid (Spain); RIKEN Nishina Center, RIKEN, Saitama (Japan); Jungclaus, A. [Instituto de Estructura de la Materia, CSIC, Madrid (Spain); Grawe, H. [GSI Helmholtzzentrum fuer Schwerionenforschung GmbH, Darmstadt (Germany); Borzov, I.N. [Kurchatov Institute, Moscow (Russian Federation); Joint Institute for Nuclear Research, Dubna (Russian Federation); Nishimura, S.; Doornenbal, P.; Soederstroem, P.A.; Baba, H.; Fukuda, N.; Inabe, N.; Isobe, T.; Kameda, D.; Kubo, T.; Shimizu, Y.; Suzuki, H.; Takeda, H.; Watanabe, H. [RIKEN Nishina Center, RIKEN, Saitama (Japan); Lorusso, G. [RIKEN Nishina Center, RIKEN, Saitama (Japan); National Physical Laboratory, NPL, Teddington, Middlesex (United Kingdom); University of Surrey, Department of Physics, Guildford (United Kingdom); Simpson, G.S.; Drouet, F. [LPSC, Universite Joseph Fourier Grenoble 1, CNRS/IN2P3, Institut National Polytechnique de Grenoble, Grenoble Cedex (France); Sumikama, T. [Tohoku University, Department of Physics, Sendai, Miyagi (Japan); Xu, Z.Y.; Niikura, M. [University of Tokyo, Department of Physics, Tokyo (Japan); Browne, F. [RIKEN Nishina Center, RIKEN, Saitama (Japan); University of Brighton, School of Computing, Engineering and Mathematics, Brighton (United Kingdom); Gernhaeuser, R.; Steiger, K.; Muecher, D. [Technische Universitaet Muenchen, Physik Department E12, Garching (Germany); Gey, G. [RIKEN Nishina Center, RIKEN, Saitama (Japan); LPSC, Universite Joseph Fourier Grenoble 1, CNRS/IN2P3, Institut National Polytechnique de Grenoble, Grenoble Cedex (France); Institut Laue-Langevin, B.P. 156, Grenoble Cedex 9 (France); Jung, H.S. [Chung-Ang University, Department of Physics, Seoul (Korea, Republic of); Kim, G.D.; Kwon, Y.K. [Institute for Basic Science, Rare Isotope Science Project, Daejeon (Korea, Republic of); Kim, Y.K. [Institute for Basic Science, Rare Isotope Science Project, Daejeon (Korea, Republic of); Hanyang University, Department of Nuclear Engineering, Seoul (Korea, Republic of); Kojouharov, I.; Kurz, N.; Schaffner, H. [Joint Institute for Nuclear Research, Dubna (Russian Federation); Li, Z. [Peking University, School of Physics and State key Laboratory of Nuclear Physics and Technology, Beijing (China); Sakurai, H. [RIKEN Nishina Center, RIKEN, Saitama (Japan); University of Tokyo, Department of Physics, Tokyo (Japan); Vajta, Zs. [RIKEN Nishina Center, RIKEN, Saitama (Japan); MTA Atomki, P.O. Box 51, Debrecen (Hungary); Wu, J. [RIKEN Nishina Center, RIKEN, Saitama (Japan); Peking University, School of Physics and State key Laboratory of Nuclear Physics and Technology, Beijing (China); Yagi, A.; Nishibata, H.; Odahara, A. [Osaka University, Department of Physics, Toyonaka (Japan); Yoshinaga, K. [Tokyo University of Science, Department of Physics, Faculty of Science and Technology, Noda, Chiba (Japan); Benzoni, G. [INFN, Sezione di Milano, Milano (Italy); Boenig, S.; Ilieva, S.; Kroell, T. [Technische Universitaet Darmstadt, Institut fuer Kernphysik, Darmstadt (Germany); Chae, K.Y. [Sungkyunkwan University, Department of Physics, Suwon (Korea, Republic of); Coraggio, L.; Gargano, A. [Complesso Universitario di Monte S. Angelo, Istituto Nazionale di Fisica Nucleare, Napoli (Italy); Daugas, J.M. [CEA, DAM, DIF, Arpajon cedex (France); Gadea, A.; Montaner-Piza, A. [CSIC-Univ. of Valencia, Instituto de Fisica Corpuscular, Paterna (Spain); Itaco, N. [Seconda Universita di Napoli, Dipartimento di Matematica e Fisica, Caserta (Italy); Kondev, F.G. [Argonne National Laboratory, Nuclear Engineering Division, Argonne, IL (United States); Lane, G.J. [Australian National University, Department of Nuclear Physics, Research School of Physical Sciences and Engineering, Canberra (Australia); Moschner, K.; Wendt, A. [University of Cologne, IKP, Cologne (Germany); Naqvi, F. [Yale University, Wright Nuclear Structure Laboratory, New Haven, CT (United States); Orlandi, R. [K.U. Leuven, Instituut voor Kern- en StralingsFysica, Heverlee (Belgium); Japan Atomic Energy Agency, Advanced Science Research Center, Tokai, Ibaraki (Japan); Patel, Z.; Podolyak, Zs. [University of Surrey, Department of Physics, Guildford (United Kingdom)

2016-11-15

The β decay of the N = 83 nucleus {sup 131}Cd has been studied at the RIBF facility at the RIKEN Nishina Center. The main purpose of the study was to identify the position of the 1p{sub 3/2} and 0f{sub 5/2} proton-hole states and the energies of core-excited configurations in the semi-magic nucleus {sup 131}In. From the radiation emitted following the β decay, a level scheme of {sup 131}In was established and the β feeding to each excited state determined. Similarities between the single-particle transitions observed in the β decays of the N = 83 isotones {sup 132}In and {sup 131}Cd are discussed. Finally the excitation energies of several core-excited configurations in {sup 131}In are compared to QRPA and shell-model calculations. (orig.)

Quantum Hooke's Law to Classify Pulse Laser Induced Ultrafast Melting

Science.gov (United States)

Hu, Hao; Ding, Hepeng; Liu, Feng

2015-02-01

Ultrafast crystal-to-liquid phase transition induced by femtosecond pulse laser excitation is an interesting material's behavior manifesting the complexity of light-matter interaction. There exist two types of such phase transitions: one occurs at a time scale shorter than a picosecond via a nonthermal process mediated by electron-hole plasma formation; the other at a longer time scale via a thermal melting process mediated by electron-phonon interaction. However, it remains unclear what material would undergo which process and why? Here, by exploiting the property of quantum electronic stress (QES) governed by quantum Hooke's law, we classify the transitions by two distinct classes of materials: the faster nonthermal process can only occur in materials like ice having an anomalous phase diagram characterized with dTm/dP < 0, where Tm is the melting temperature and P is pressure, above a high threshold laser fluence; while the slower thermal process may occur in all materials. Especially, the nonthermal transition is shown to be induced by the QES, acting like a negative internal pressure, which drives the crystal into a ``super pressing'' state to spontaneously transform into a higher-density liquid phase. Our findings significantly advance fundamental understanding of ultrafast crystal-to-liquid phase transitions, enabling quantitative a priori predictions.

BEC-BCS-laser crossover in Coulomb-correlated electron-hole-photon systems

International Nuclear Information System (INIS)

Yamaguchi, M; Kamide, K; Ogawa, T; Yamamoto, Y

2012-01-01

Many-body features caused by Coulomb correlations are of great importance for understanding phenomena pertaining to polariton systems in semiconductor microcavities, i.e. electron-hole-photon systems. Remarkable many-body effects are shown to exist in both thermal-equilibrium phases and non-equilibrium lasing states. We then show a unified framework for connecting the thermal-equilibrium and the non-equilibrium steady states based on a non-equilibrium Green's function approach. Bose-Einstein condensate (BEC)-Bardeen-Cooper-Schrieffer (BCS)-laser crossovers are investigated by using this approach. (paper)

The 40Ar/39Ar and K/Ar dating of lavas from the Hilo 1-km core hole, Hawaii Scientific Drilling Project

Science.gov (United States)

Sharp, W.D.; Turrin, B.D.; Renne, P.R.; Lanphere, M.A.

1996-01-01

Mauna Kea lava flows cored in the HilIo hole range in age from <200 ka to about 400 ka based on 40Ar/39Ar incremental heating and K-Ar analyses of 16 groundmass samples and one coexisting plagioclase. The lavas, all subaerially deposited, include a lower section consisting only of tholeiitic basalts and an upper section of interbedded alkalic, transitional tholeiitic, and tholeiitic basalts. The lower section has yielded predominantly complex, discordant 40Ar/39Ar age spectra that result from mobility of 40Ar and perhaps K, the presence of excess 40Ar, and redistribution of 39Ar by recoil. Comparison of K-Ar ages with 40Ar/39Ar integrated ages indicates that some of these samples have also lost 39Ar. Nevertheless, two plateau ages of 391 ?? 40 and 400 ?? 26 ka from deep in the hole, combined with data from the upper section, show that the tholeiitic section accumulated at an average rate of about 7 to 8 m/kyr and has an mean recurrence interval of 0.5 kyr/flow unit. Samples from the upper section yield relatively precise 40Ar/39Ar plateau and isotope correlation ages of 326 ?? 23, 241 ?? 5, 232 ?? 4, and 199 ?? 9 ka for depths of -415.7 m to -299.2 m. Within their uncertainty, these ages define a linear relationship with depth, with an average accumulation rate of 0.9 m/kyr and an average recurrence interval of 4.8 kyr/flow unit. The top of the Mauna Kea sequence at -280 m must be older than the plateau age of 132 ?? 32 ka, obtained for the basal Mauna Loa flow in the corehole. The upward decrease in lava accumulation rate is a consequence of the decreasing magma supply available to Mauna Kea as it rode the Pacific plate away from its magma source, the Hawaiian mantle plume. The age-depth relation in the core hole may be used to test and refine models that relate the growth of Mauna Kea to the thermal and compositional structure of the mantle plume.

A PSF-Shape-Based Beamforming Strategy for Robust 2D Motion Estimation in Ultrafast Data

OpenAIRE

Anne E. C. M. Saris; Stein Fekkes; Maartje M. Nillesen; Hendrik H. G. Hansen; Chris L. de Korte

2018-01-01

This paper presents a framework for motion estimation in ultrafast ultrasound data. It describes a novel approach for determining the sampling grid for ultrafast data based on the system’s point-spread-function (PSF). As a consequence, the cross-correlation functions (CCF) used in the speckle tracking (ST) algorithm will have circular-shaped peaks, which can be interpolated using a 2D interpolation method to estimate subsample displacements. Carotid artery wall motion and parabolic blood flow...

Avant-Garde Ultrafast Laser Writing

Directory of Open Access Journals (Sweden)

Kazansky P. G.

2013-11-01

Full Text Available Ultrafast laser processing of transparent materials reveals new phenomena. Reviewed, are recent demonstrations of 5D optical memory, vortex polarization and Airy beam converters employing self-assembled nanostructuring, ultrafast laser calligraphy and polarization writing control using pulses with tilted front.

Ultrafast nonlinear optics

CERN Document Server

Leburn, Christopher; Reid, Derryck

2013-01-01

The field of ultrafast nonlinear optics is broad and multidisciplinary, and encompasses areas concerned with both the generation and measurement of ultrashort pulses of light, as well as those concerned with the applications of such pulses. Ultrashort pulses are extreme events – both in terms of their durations, and also the high peak powers which their short durations can facilitate. These extreme properties make them powerful experiment tools. On one hand, their ultrashort durations facilitate the probing and manipulation of matter on incredibly short timescales. On the other, their ultrashort durations can facilitate high peak powers which can drive highly nonlinear light-matter interaction processes. Ultrafast Nonlinear Optics covers a complete range of topics, both applied and fundamental in nature, within the area of ultrafast nonlinear optics. Chapters 1 to 4 are concerned with the generation and measurement of ultrashort pulses. Chapters 5 to 7 are concerned with fundamental applications of ultrasho...

Edge turbulence effect on ultra-fast swept reflectometry core measurements in tokamak plasmas

Science.gov (United States)

Zadvitskiy, G. V.; Heuraux, S.; Lechte, C.; Hacquin, S.; Sabot, R.

2018-02-01

Ultra-fast frequency-swept reflectometry (UFSR) enables one to provide information about the turbulence radial wave-number spectrum and perturbation amplitude with good spatial and temporal resolutions. However, a data interpretation of USFR is quiet tricky. An iterative algorithm to solve this inverse problem was used in past works, Gerbaud (2006 Rev. Sci. Instrum. 77 10E928). For a direct solution, a fast 1D Helmholtz solver was used. Two-dimensional effects are strong and should be taken into account during data interpretation. As 2D full-wave codes are still too time consuming for systematic application, fast 2D approaches based on the Born approximation are of prime interest. Such methods gives good results in the case of small turbulence levels. However in tokamak plasmas, edge turbulence is usually very strong and can distort and broaden the probing beam Sysoeva et al (2015 Nucl. Fusion 55 033016). It was shown that this can change reflectometer phase response from the plasma core. Comparison between 2D full wave computation and the simplified Born approximation was done. The approximated method can provide a right spectral shape, but it is unable to describe a change of the spectral amplitude with an edge turbulence level. Computation for the O-mode wave with the linear density profile in the slab geometry and for realistic Tore-Supra density profile, based on the experimental data turbulence amplitude and spectrum, were performed to investigate the role of strong edge turbulence. It is shown that the spectral peak in the signal amplitude variation spectrum which rises with edge turbulence can be a signature of strong edge turbulence. Moreover, computations for misaligned receiving and emitting antennas were performed. It was found that the signal amplitude variation peak changes its position with a receiving antenna poloidal displacement.

Petrologic studies of drill cores USW-G2 and UE25b-1H, Yucca Mountain, Nevada

International Nuclear Information System (INIS)

Caporuscio, F.; Vaniman, D.; Bish, D.; Broxton, D.; Arney, B.; Heiken, G.; Byers, F.; Gooley, R.; Semarge, E.

1982-07-01

The tuffs of the Nevada Test Site are currently under investigation as a possible deep geologic site for high-level radioactive waste disposal. This report characterizes tuff retrieved in core from two drill holes, USW-G2 and UE25b-1H, at the Yucca Mountain block. The USW-G2 drill core is from the northernmost extent of the block, whereas UE25b-1H is adjacent to an earlier drill hole, UE25a-1. The drill cores USW-G2 and UE25b-1H bottomed at 6000 and 4200 ft, respectively. Petrographic and x-ray diffraction studies of the two drill cores are presented in this report and indicate that tuffs (composed primarily of variably welded ash flows) are partially recrystallized to secondary minerals. Correlations of stratigraphy are also made with previous drill cores from Yucca Mountain

Core drilling provides information about Santa Fe Group aquifer system beneath Albuquerque's West Mesa

Science.gov (United States)

Allen, B.D.; Connell, S.D.; Hawley, J.W.; Stone, B.D.

1998-01-01

Core samples from the upper ???1500 ft of the Santa Fe Group in the Albuquerque West Mesa area provide a first-hand look at the sediments and at subsurface stratigraphic relationships in this important part of the basin-fill aquifer system. Two major hydrostratigraphic subunits consisting of a lower coarse-grained, sandy interval and an overlying fine-grained, interbedded silty sand and clay interval lie beneath the water table at the 98th St core hole. Borehole electrical conductivity measurements reproduce major textural changes observed in the recovered cores and support subsurface correlations of hydrostratigraphic units in the Santa Fe Group aquifer system based on geophysical logs. Comparison of electrical logs from the core hole and from nearby city wells reveals laterally consistent lithostratigraphic patterns over much of the metropolitan area west of the Rio Grande that may be used to delineate structural and related stratigraphic features that have a direct bearing on the availability of ground water.

Recovery and Lithologic Analysis of Sediment from Hole UT-GOM2-1-H002, Green Canyon 955, Northern Gulf of Mexico

Science.gov (United States)

Kinash, N.; Cook, A.; Sawyer, D.; Heber, R.

2017-12-01

In May 2017 the University of Texas led a drilling and pressure coring expedition in the northern Gulf of Mexico, UT-GOM2-01. The holes were located in Green Canyon Block 955, where the Gulf of Mexico Joint Industry Project Leg II identified an approximately 100m thick hydrate-filled course-grained levee unit in 2009. Two separate wells were drilled into this unit: Holes H002 and H005. In Hole H002, a cutting shoe drill bit was used to collect the pressure cores, and only 1 of the 8 cores collected was pressurized during recovery. The core recovery in Hole H002 was generally poor, about 34%, while the only pressurized core had 45% recovery. In Hole H005, a face bit was used during pressure coring where 13 cores were collected and 9 cores remained pressurized. Core recovery in Hole H005 was much higher, at about 75%. The type of bit was not the only difference between the holes, however. Drilling mud was used throughout the drilling and pressure coring of Hole H002, while only seawater was used during the first 80m of pressure cores collected in Hole H005. Herein we focus on lithologic analysis of Hole H002 with the goal of documenting and understanding core recovery in Hole H002 to compare with Hole H005. X-ray Computed Tomography (XCT) images were collected by Geotek on pressurized cores, mostly from Hole H005, and at Ohio State on unpressurized cores, mostly from Hole H002. The XCT images of unpressurized cores show minimal sedimentary structures and layering, unlike the XCT images acquired on the pressurized, hydrate-bearing cores. Only small sections of the unpressurized cores remained intact. The unpressurized cores appear to have two prominent facies: 1) silt that did not retain original sedimentary fabric and often was loose within the core barrel, and 2) dense mud sections with some sedimentary structures and layering present. On the XCT images, drilling mud appears to be concentrated on the sides of cores, but also appears in layers and fractures within

Momentum distributions for two-electron systems: electron correlation and the Coulomb hole

International Nuclear Information System (INIS)

Banyard, K.E.; Reed, C.E.

1978-01-01

By evaluating the distribution function f(p 12 ), where p 12 ) in momentum space can be investigated. difference[p 1 - p 2 ] the concept of a Coulomb hole Δf(p 12 ) in momentum space can be investigated. Results are presented for the isoelectronic systems H - , He and Li + . The electron correlation within each CI wavefunction was analysed into its radial and angular components so that the structure and composition of Δf(p 12 ) could be assessed. The two-particle momentum radial density distribution and several two-particle expectation quantities are also examined. The present findings indicate, that in momentum space, the radial components of correlation produce effects characteristic of total correlation in position space whereas, by contrast, angular correlation creates an opposite effect. Thus the shape and formation of Δf(p 12 ) proves to be considerably more complex than that found for its counterpart in position space. The results also reveal a noticeable change in the relative importance of the components of correlation as the momentum increases. (author)

Probing ultrafast carrier tunneling dynamics in individual quantum dots and molecules

Energy Technology Data Exchange (ETDEWEB)

Mueller, Kai; Bechtold, Alexander; Kaldewey, Timo; Zecherle, Markus; Wildmann, Johannes S.; Bichler, Max; Abstreiter, Gerhard; Finley, Jonathan J. [Walter Schottky Institut and Physik-Department, Technische Universitaet Muenchen, Am Coulombwall 4, 85748, Garching (Germany); Ruppert, Claudia; Betz, Markus [Experimentelle Physik 2, TU Dortmund, 44221, Dortmund (Germany); Krenner, Hubert J. [Lehrstuhl fuer Experimentalphysik 1 and Augsburg Centre for Innovative Technologies (ACIT), Universitaet Augsburg, Universitaetsstr 1, 86159, Augsburg (Germany); Villas-Boas, Jose M. [Instituto de Fisica, Universidade Federal de Uberlandia, 38400-902, Uberlandia, MG (Brazil)

2013-02-15

Ultrafast pump-probe spectroscopy is employed to directly monitor the tunneling of charge carriers from single and vertically coupled quantum dots and probe intra-molecular dynamics. Immediately after resonant optical excitation, several peaks are observed in the pump-probe spectrum arising from Coulomb interactions between the photogenerated charge carriers. The influence of few-Fermion interactions in the photoexcited system and the temporal evolution of the optical response is directly probed in the time domain. In addition, the tunneling times for electrons and holes from the QD nanostructure are independently determined. In polarization resolved measurements, near perfect Pauli-spin blockade is observed in the spin-selective absorption spectrum as well as stimulated emission. While electron and hole tunneling from single quantum dots is shown to be well explained by the WKB formalism, for coupled quantum dots pronounced resonances in the electron tunneling rate are observed arising from elastic and inelastic electron tunneling between the different dots. (copyright 2012 by WILEY-VCH Verlag GmbH and Co. KGaA, Weinheim)

Selection bias in dynamically measured supermassive black hole samples: scaling relations and correlations between residuals in semi-analytic galaxy formation models

Science.gov (United States)

Barausse, Enrico; Shankar, Francesco; Bernardi, Mariangela; Dubois, Yohan; Sheth, Ravi K.

2017-07-01

Recent work has confirmed that the scaling relations between the masses of supermassive black holes and host-galaxy properties such as stellar masses and velocity dispersions may be biased high. Much of this may be caused by the requirement that the black hole sphere of influence must be resolved for the black hole mass to be reliably estimated. We revisit this issue with a comprehensive galaxy evolution semi-analytic model. Once tuned to reproduce the (mean) correlation of black hole mass with velocity dispersion, the model cannot account for the correlation with stellar mass. This is independent of the model's parameters, thus suggesting an internal inconsistency in the data. The predicted distributions, especially at the low-mass end, are also much broader than observed. However, if selection effects are included, the model's predictions tend to align with the observations. We also demonstrate that the correlations between the residuals of the scaling relations are more effective than the relations themselves at constraining models for the feedback of active galactic nuclei (AGNs). In fact, we find that our model, while in apparent broad agreement with the scaling relations when accounting for selection biases, yields very weak correlations between their residuals at fixed stellar mass, in stark contrast with observations. This problem persists when changing the AGN feedback strength, and is also present in the hydrodynamic cosmological simulation Horizon-AGN, which includes state-of-the-art treatments of AGN feedback. This suggests that current AGN feedback models are too weak or simply not capturing the effect of the black hole on the stellar velocity dispersion.

Direct Observation of Ultrafast Hole Injection from Lead Halide Perovskite by Differential Transient Transmission Spectroscopy.

Science.gov (United States)

Ishioka, Kunie; Barker, Bobby G; Yanagida, Masatoshi; Shirai, Yasuhiro; Miyano, Kenjiro

2017-08-17

Efficient charge separation at the interfaces of the perovskite with the carrier transport layers is crucial for perovskite solar cells to achieve high power conversion efficiency. We present a systematic experimental study on the hole injection dynamics from MAPbI 3 perovskite to three typical hole transport materials (HTMs). We extract the carrier dynamics directly related to the hole injection by employing a pump light with short absorption depth and comparing the transient transmission signals excited on the two sides of the sample. The differential transmission signals reveal the hole injections to PTAA and PEDOT:PSS to be complete within 1 and 2 ps, respectively, and that to NiO x to exhibit an additional slow process on a 40 ps time scale. The obtained injection dynamics are discussed in comparison with the device performance of the solar cells containing the same MAPbI 3 /HTM interfaces.

Ultrafast dynamics during the photoinduced phase transition in VO2

Science.gov (United States)

Wegkamp, Daniel; Stähler, Julia

2015-12-01

The phase transition of VO2 from a monoclinic insulator to a rutile metal, which occurs thermally at TC = 340 K, can also be driven by strong photoexcitation. The ultrafast dynamics during this photoinduced phase transition (PIPT) have attracted great scientific attention for decades, as this approach promises to answer the question of whether the insulator-to-metal (IMT) transition is caused by electronic or crystallographic processes through disentanglement of the different contributions in the time domain. We review our recent results achieved by femtosecond time-resolved photoelectron, optical, and coherent phonon spectroscopy and discuss them within the framework of a selection of latest, complementary studies of the ultrafast PIPT in VO2. We show that the population change of electrons and holes caused by photoexcitation launches a highly non-equilibrium plasma phase characterized by enhanced screening due to quasi-free carriers and followed by two branches of non-equilibrium dynamics: (i) an instantaneous (within the time resolution) collapse of the insulating gap that precedes charge carrier relaxation and significant ionic motion and (ii) an instantaneous lattice potential symmetry change that represents the onset of the crystallographic phase transition through ionic motion on longer timescales. We discuss the interconnection between these two non-thermal pathways with particular focus on the meaning of the critical fluence of the PIPT in different types of experiments. Based on this, we conclude that the PIPT threshold identified in optical experiments is most probably determined by the excitation density required to drive the lattice potential change rather than the IMT. These considerations suggest that the IMT can be driven by weaker excitation, predicting a transiently metallic, monoclinic state of VO2 that is not stabilized by the non-thermal structural transition and, thus, decays on ultrafast timescales.

Investigation on properties of ultrafast switching in a bulk gallium arsenide avalanche semiconductor switch

International Nuclear Information System (INIS)

Hu, Long; Su, Jiancang; Ding, Zhenjie; Hao, Qingsong; Yuan, Xuelin

2014-01-01

Properties of ultrafast switching in a bulk gallium arsenide (GaAs) avalanche semiconductor switch based on semi-insulating wafer, triggered by an optical pulse, were analyzed using physics-based numerical simulations. It has been demonstrated that when a voltage with amplitude of 5.2 kV is applied, after an exciting optical pulse with energy of 1 μJ arrival, the structure with thickness of 650 μm reaches a high conductivity state within 110 ps. Carriers are created due to photons absorption, and electrons and holes drift to anode and cathode terminals, respectively. Static ionizing domains appear both at anode and cathode terminals, and create impact-generated carriers which contribute to the formation of electron-hole plasma along entire channel. When the electric field in plasma region increases above the critical value (∼4 kV/cm) at which the electrons drift velocity peaks, a domain comes into being. An increase in carrier concentration due to avalanche multiplication in the domains reduces the domain width and results in the formation of an additional domain as soon as the field outside the domains increases above ∼4 kV/cm. The formation and evolution of multiple powerfully avalanching domains observed in the simulations are the physical reasons of ultrafast switching. The switch exhibits delayed breakdown with the characteristics affected by biased electric field, current density, and optical pulse energy. The dependence of threshold energy of the exciting optical pulse on the biased electric field is discussed

Intermediate-Mass Black Holes

Science.gov (United States)

Miller, M. Coleman; Colbert, E. J. M.

2004-01-01

The mathematical simplicity of black holes, combined with their links to some of the most energetic events in the universe, means that black holes are key objects for fundamental physics and astrophysics. Until recently, it was generally believed that black holes in nature appear in two broad mass ranges: stellar-mass (M~3 20 M⊙), which are produced by the core collapse of massive stars, and supermassive (M~106 1010 M⊙), which are found in the centers of galaxies and are produced by a still uncertain combination of processes. In the last few years, however, evidence has accumulated for an intermediate-mass class of black holes, with M~102 104 M⊙. If such objects exist they have important implications for the dynamics of stellar clusters, the formation of supermassive black holes, and the production and detection of gravitational waves. We review the evidence for intermediate-mass black holes and discuss future observational and theoretical work that will help clarify numerous outstanding questions about these objects.

Ultrafast quenching of tryptophan fluorescence in proteins: Interresidue and intrahelical electron transfer

Energy Technology Data Exchange (ETDEWEB)

Qiu Weihong; Li Tanping; Zhang Luyuan; Yang Yi; Kao Yating; Wang Lijuan [Department of Physics, Chemistry, and Biochemistry, Program of Biophysics, Chemical Physics, and Biochemistry, Ohio State University, Columbus, OH 43210 (United States); Zhong Dongping [Department of Physics, Chemistry, and Biochemistry, Program of Biophysics, Chemical Physics, and Biochemistry, Ohio State University, Columbus, OH 43210 (United States)], E-mail: dongping@mps.ohio-state.edu

2008-06-23

Quenching of tryptophan fluorescence in proteins has been critical to the understanding of protein dynamics and enzyme reactions using tryptophan as a molecular optical probe. We report here our systematic examinations of potential quenching residues with more than 40 proteins. With site-directed mutation, we placed tryptophan to desired positions or altered its neighboring residues to screen quenching groups among 20 amino acid residues and of peptide backbones. With femtosecond resolution, we observed the ultrafast quenching dynamics within 100 ps and identified two ultrafast quenching groups, the carbonyl- and sulfur-containing residues. The former is glutamine and glutamate residues and the later is disulfide bond and cysteine residue. The quenching by the peptide-bond carbonyl group as well as other potential residues mostly occurs in longer than 100 ps. These ultrafast quenching dynamics occur at van der Waals distances through intraprotein electron transfer with high directionality. Following optimal molecular orbital overlap, electron jumps from the benzene ring of the indole moiety in a vertical orientation to the LUMO of acceptor quenching residues. Molecular dynamics simulations were invoked to elucidate various correlations of quenching dynamics with separation distances, relative orientations, local fluctuations and reaction heterogeneity. These unique ultrafast quenching pairs, as recently found to extensively occur in high-resolution protein structures, may have significant biological implications.

Neogene and Quaternary geology of a stratigraphic test hole on Horn Island, Mississippi Sound

Science.gov (United States)

Gohn, Gregory S.; Brewster-Wingard, G. Lynn; Cronin, Thomas M.; Edwards, Lucy E.; Gibson, Thomas G.; Rubin, Meyer; Willard, Debra A.

1996-01-01

During April and May, 1991, the U.S. Geological Survey (USGS) drilled a 510-ft-deep, continuously cored, stratigraphic test hole on Horn Island, Mississippi Sound, as part of a field study of the Neogene and Quaternary geology of the Mississippi coastal area. The USGS drilled two new holes at the Horn Island site. The first hole was continuously cored to a depth of 510 ft; coring stopped at this depth due to mechanical problems. To facilitate geophysical logging, an unsampled second hole was drilled to a depth of 519 ft at the same location.

The response of relativistic outflowing gas to the inner accretion disk of a black hole.

Science.gov (United States)

Parker, Michael L; Pinto, Ciro; Fabian, Andrew C; Lohfink, Anne; Buisson, Douglas J K; Alston, William N; Kara, Erin; Cackett, Edward M; Chiang, Chia-Ying; Dauser, Thomas; De Marco, Barbara; Gallo, Luigi C; Garcia, Javier; Harrison, Fiona A; King, Ashley L; Middleton, Matthew J; Miller, Jon M; Miniutti, Giovanni; Reynolds, Christopher S; Uttley, Phil; Vasudevan, Ranjan; Walton, Dominic J; Wilkins, Daniel R; Zoghbi, Abderahmen

2017-03-01

The brightness of an active galactic nucleus is set by the gas falling onto it from the galaxy, and the gas infall rate is regulated by the brightness of the active galactic nucleus; this feedback loop is the process by which supermassive black holes in the centres of galaxies may moderate the growth of their hosts. Gas outflows (in the form of disk winds) release huge quantities of energy into the interstellar medium, potentially clearing the surrounding gas. The most extreme (in terms of speed and energy) of these-the ultrafast outflows-are the subset of X-ray-detected outflows with velocities higher than 10,000 kilometres per second, believed to originate in relativistic (that is, near the speed of light) disk winds a few hundred gravitational radii from the black hole. The absorption features produced by these outflows are variable, but no clear link has been found between the behaviour of the X-ray continuum and the velocity or optical depth of the outflows, owing to the long timescales of quasar variability. Here we report the observation of multiple absorption lines from an extreme ultrafast gas flow in the X-ray spectrum of the active galactic nucleus IRAS 13224-3809, at 0.236 ± 0.006 times the speed of light (71,000 kilometres per second), where the absorption is strongly anti-correlated with the emission of X-rays from the inner regions of the accretion disk. If the gas flow is identified as a genuine outflow then it is in the fastest five per cent of such winds, and its variability is hundreds of times faster than in other variable winds, allowing us to observe in hours what would take months in a quasar. We find X-ray spectral signatures of the wind simultaneously in both low- and high-energy detectors, suggesting a single ionized outflow, linking the low- and high-energy absorption lines. That this disk wind is responding to the emission from the inner accretion disk demonstrates a connection between accretion processes occurring on very different

Influence of the core-hole effect on optical properties of magnesium oxide (MgO) near the Mg L-edge region.

Science.gov (United States)

Sinha, Mangalika; Modi, Mohammed H; Ghosh, Haranath; Yadav, P K; Gupta, R K

2018-05-01

The influence of the core-hole effect on optical properties of magnesium oxide (MgO) is established through experimental determination of optical constants and first-principles density functional theory studies. Optical constants (δ and β) of MgO thin film are measured in the spectral region 40-300 eV using reflectance spectroscopy techniques at the Indus-1 synchrotron radiation source. The obtained optical constants show strong core exciton features near the Mg L-edge region, causing significant mismatch with Henke's tabulated values. On comparing the experimentally obtained optical constants with Henke's tabulated values, an edge shift of ∼3.0 eV is also observed. Distinct evidence of effects of core exciton on optical constants (δ and β) in the near Mg L-edge absorption spectra are confirmed through first-principles simulations.

Ultrafast Interfacial Electron and Hole Transfer from CsPbBr3 Perovskite Quantum Dots.

Science.gov (United States)

Wu, Kaifeng; Liang, Guijie; Shang, Qiongyi; Ren, Yueping; Kong, Degui; Lian, Tianquan

2015-10-14

Recently reported colloidal lead halide perovskite quantum dots (QDs) with tunable photoluminescence (PL) wavelengths covering the whole visible spectrum and exceptionally high PL quantum yields (QYs, 50-90%) constitute a new family of functional materials with potential applications in light-harvesting and -emitting devices. By transient absorption spectroscopy, we show that the high PL QYs (∼79%) can be attributed to negligible electron or hole trapping pathways in CsPbBr3 QDs: ∼94% of lowest excitonic states decayed with a single-exponential time constant of 4.5 ± 0.2 ns. Furthermore, excitons in CsPbBr3 QDs can be efficiently dissociated in the presence of electron or hole acceptors. The half-lives of electron transfer (ET) to benzoquinone and subsequent charge recombination are 65 ± 5 ps and 2.6 ± 0.4 ns, respectively. The half-lives for hole transfer (HT) to phenothiazine and the subsequent charge recombination are 49 ± 6 ps and 1.0 ± 0.2 ns, respectively. The lack of electron and hole traps and fast interfacial ET and HT rates are key properties that may enable the development of efficient lead halide perovskite QDs-based light-harvesting and -emitting devices.

Ultrafast THz saturable absorption in doped semiconductors at room temperature

DEFF Research Database (Denmark)

Turchinovich, Dmitry; Hoffmann, M. V.

2011-01-01

Ultrafast Phenomena XVII presents the latest advances in ultrafast science, including both ultrafast optical technology and the study of ultrafast phenomena. It covers picosecond, femtosecond and attosecond processes relevant to applications in physics, chemistry, biology, and engineering. Ultraf...

Correlation and flux tilt measurements of coupled-core reactor assemblies

International Nuclear Information System (INIS)

Harries, J.R.

1976-01-01

The systematics of coupling reactivity and time delay between cores have been investigated with a series of coupled-core assemblies on the AAEC Split-table Critical Facility. The assemblies were similar to the Universities' Training Reactor (UTR), but had graphite coupling region thickness of 450 mm, 600 mm and 800 mm. The coupling reactivity measured by both the cross-correlation of reactor noise and the flux tilt methods was stronger than for the UTRs, but showed a similar trend with core spacing. The cross-correlograms were analysed using the two-node model to derive the time delays between the cores. The time delays were compared with thermal neutron wave propagation, and found to be consistent when the time delays were added to the individual node response-function delays. (author)

Effect of Osteonecrosis Intervention Rod Versus Core Decompression Using Multiple Small Drill Holes on Early Stages of Necrosis of the Femoral Head: A Prospective Study on a Series of 60 Patients with a Minimum 1-Year-Follow-Up.

Science.gov (United States)

Miao, Haixiong; Ye, Dongping; Liang, Weiguo; Yao, Yicun

2015-01-01

The conventional CD used 10 mm drill holes associated with a lack of structural support. Thus, alternative methods such as a tantalum implant, small drill holes, and biological treatment were developed to prevent deterioration of the joint. The treatment of CD by multiple 3.2 mm drill holes could reduce the femoral neck fracture and partial weight bearing was allowed. This study was aimed to evaluate the effect of osteonecrosis intervention rod versus core decompression using multiple small drill holes on early stages of necrosis of the femoral head. From January 2011 to January 2012, 60 patients undergoing surgery for osteonecrosis with core decompression were randomly assigned into 2 groups based on the type of core decompression used: (1) a total of 30 osteonecrosis patients (with 16 hips on Steinburg stageⅠ,20 hips on Steinburg stageⅡ) were treated with a porous tantalum rod insertion. The diameter of the drill hole for the intervention rod was 10mm.(2) a total of 30 osteonecrosis patients (with 14 hips on Steinburg stageⅠ,20 hips on Steinburg stageⅡ) were treated with core decompression using five drill holes on the lateral femur, the diameter of the hole was 3.2 mm. The average age of the patient was 32.6 years (20-45 years) and the average time of follow-up was 25.6 months (12- 28 months) in the rod implanted group. The average age of the patient was 35.2 years (22- 43 years) and the average time of follow-up was 26.3 months (12-28 months) in the small drill holes group. The average of surgical time was 40 min, and the mean volume of blood loss was 30 ml in both surgical groups. The average of Harris score was improved from 56.2 ± 7.1 preoperative to 80.2 ± 11.4 at the last follow-up in the rod implanted group (p holes group (pholes group. No significant difference was observed in radiographic stage between the two groups. There was no favourable result on the outcome of a tantalum intervention implant compared to multiple small drill holes. CD via

Regular black holes: electrically charged solutions, Reissner-Nordstroem outside a De Sitter core

Energy Technology Data Exchange (ETDEWEB)

Lemos, Jose P.S. [Universidade Tecnica de Lisboa (CENTRA/IST/UTL) (Portugal). Instituto Superior Tecnico. Centro Multidisciplinar de Astrofisica; Zanchin, Vilson T. [Universidade Federal do ABC (UFABC), Santo Andre, SP (Brazil). Centro de Ciencias Naturais e Humanas

2011-07-01

Full text: The understanding of the inside of a black hole is of crucial importance in order to have the correct picture of a black hole as a whole. The singularities that lurk inside of the usual black hole solutions are things to avoid. Their substitution by a regular part is of great interest, the process generating regular black holes. In the present work regular black hole solutions are found within general relativity coupled to Maxwell's electromagnetism and charged matter. We show that there are objects which correspond to regular charged black holes, whose interior region is de Sitter, whose exterior region is Reissner-Nordstroem, and the boundary between both regions is made of an electrically charged spherically symmetric coat. There are several solutions: the regular nonextremal black holes with a null matter boundary, the regular nonextremal black holes with a timelike matter boundary, the regular extremal black holes with a timelike matter boundary, and the regular overcharged stars with a timelike matter boundary. The main physical and geometrical properties of such charged regular solutions are analyzed. (author)

Relativistic many-body XMCD theory including core degenerate effects

Science.gov (United States)

Fujikawa, Takashi

2009-11-01

A many-body relativistic theory to analyze X-ray Magnetic Circular Dichroism (XMCD) spectra has been developed on the basis of relativistic quantum electrodynamic (QED) Keldysh Green's function approach. This theoretical framework enables us to handle relativistic many-body effects in terms of correlated nonrelativistic Green's function and relativistic correction operator Q, which naturally incorporates radiation field screening and other optical field effects in addition to electron-electron interactions. The former can describe the intensity ratio of L2/L3 which deviates from the statistical weight (branching ratio) 1/2. In addition to these effects, we consider the degenerate or nearly degenerate effects of core levels from which photoelectrons are excited. In XPS spectra, for example in Rh 3d sub level excitations, their peak shapes are quite different: This interesting behavior is explained by core-hole moving after the core excitation. We discuss similar problems in X-ray absorption spectra in particular excitation from deep 2p sub levels which are degenerate in each sub levels and nearly degenerate to each other in light elements: The hole left behind is not frozen there. We derive practical multiple scattering formulas which incorporate all those effects.

Determination of three-dimensional stress orientations in the Wenchuan earthquake Fault Scientific Drilling (WFSD) hole-1: A preliminary result by anelastic strain recovery measurements of core samples

Science.gov (United States)

Cui, J.; Lin, W.; Wang, L.; Tang, Z.; Sun, D.; Gao, L.; Wang, W.

2010-12-01

A great and destructive earthquake (Ms 8.0; Mw 7.9), Wunchuan earthquake struck on the Longmen Shan foreland trust zone in Sichuan province, China on 12 May 2008 (Xu et al., 2008; Episodes, Vol.31, pp.291-301). As a rapid response scientific drilling project, Wenchuan earthquake Fault Scientific Drilling (WFSD) started on 6 November 2008 shorter than a half of year from the date of earthquake main shock. The first pilot borehole (hole-1) has been drilled to the target depth (measured depth 1201 m MD, vertical depth 1179 m) at Hongkou, Dujianyan, Sichuan and passed through the main fault of the earthquake around 589 m MD. We are trying to determine three dimensional in-situ stress states in the WFSD boreholes by a core-based method, anelastic strain recovery (ASR) method (Lin et al., 2006; Tectonophysics, Vol4.26, pp.221-238). This method has been applied in several scientific drilling projects (TCDP: Lin et al., 2007; TAO, Vol.18, pp.379-393; NanTtoSEIZE: Byrne et al., 2009; GRL, Vol.36, L23310). These applications confirm the validity of using the ASR technique in determining in situ stresses by using drilled cores. We collected total 15 core samples in a depth range from 340 m MD to 1180 m MD, approximately for ASR measurements. Anelastic normal strains, measured every ten minutes in nine directions, including six independent directions, were used to calculate the anelastic strain tensors. The data of the ASR tests conducted at hole-1 is still undergoing analysis. As a tentative perspective, more than 10 core samples showed coherent strain recovery over one - two weeks. However, 2 or 3 core samples cannot be re-orientated to the global system. It means that we cannot rink the stress orientation determined by the core samples to geological structure. Unfortunately, a few core samples showed irregular strain recovery and were not analyzed further. The preliminary results of ASR tests at hole-1 show the stress orientations and stress regime changes a lot with the

Generation of mega-electron-volt electron beams by an ultrafast intense laser pulse

International Nuclear Information System (INIS)

Wang Xiaofang; Saleh, Ned; Krishnan, Mohan; Wang Haiwen; Backus, Sterling; Murnane, Margaret; Kapteyn, Henry; Umstadter, Donald; Wang Quandong; Shen Baifei

2003-01-01

Mega-electron-volt (MeV) electron emission from the interaction of an ultrafast (τ∼29 fs), intense (>10 18 W/cm 2 ) laser pulse with underdense plasmas has been studied. A beam of MeV electrons with a divergence angle as small as 1 deg. is observed in the forward direction, which is correlated with relativistic filamentation of the laser pulse in plasmas. A novel net-energy-gain mechanism is proposed for electron acceleration resulting from the relativistic filamentation and beam breakup. These results suggest an approach for generating a beam of femtosecond, MeV electrons at a kilohertz repetition rate with a compact ultrafast intense laser system

Ultra-fast movies of thin-film laser ablation

Science.gov (United States)

Domke, Matthias; Rapp, Stephan; Schmidt, Michael; Huber, Heinz P.

2012-11-01

Ultra-short-pulse laser irradiation of thin molybdenum films from the glass substrate side initiates an intact Mo disk lift off free from thermal effects. For the investigation of the underlying physical effects, ultra-fast pump-probe microscopy is used to produce stop-motion movies of the single-pulse ablation process, initiated by a 660-fs laser pulse. The ultra-fast dynamics in the femtosecond and picosecond ranges are captured by stroboscopic illumination of the sample with an optically delayed probe pulse of 510-fs duration. The nanosecond and microsecond delay ranges of the probe pulse are covered by an electronically triggered 600-ps laser. Thus, the setup enables an observation of general laser ablation processes from the femtosecond delay range up to the final state. A comparison of time- and space-resolved observations of film and glass substrate side irradiation of a 470-nm molybdenum layer reveals the driving mechanisms of the Mo disk lift off initiated by glass-side irradiation. Observations suggest that a phase explosion generates a liquid-gas mixture in the molybdenum/glass interface about 10 ps after the impact of the pump laser pulse. Then, a shock wave and gas expansion cause the molybdenum layer to bulge, while the enclosed liquid-gas mixture cools and condenses at delay times in the 100-ps range. The bulging continues for approximately 20 ns, when an intact Mo disk shears and lifts off at a velocity of above 70 m/s. As a result, the remaining hole is free from thermal effects.

Ultrabroadband polarization splitter based on three-core photonic crystal fiber with a modulation core.

Science.gov (United States)

Zhao, Tongtong; Lou, Shuqin; Wang, Xin; Zhou, Min; Lian, Zhenggang

2016-08-10

We design an ultrabroadband polarization splitter based on three-core photonic crystal fiber (PCF). A modulation core and two fluorine-doped cores are introduced to achieve an ultrawide bandwidth. The properties of three-core PCF are modeled by using the full-vector finite element method along with the full-vector beam propagation method. Numerical results demonstrate that an ultrabroadband splitter with 320 nm bandwidth with an extinction ratio as low as -20  dB can be achieved by using 52.8 mm long three-core PCF. This splitter also has high compatibility with standard single-mode fibers as the input and output ports due to low splicing loss of 0.02 dB. All the air holes in the proposed structure are circular holes and arranged in a triangular lattice that makes it easy to fabricate.

Water-core Fresnel fiber

NARCIS (Netherlands)

Martelli, C.; Canning, J.; Lyytikainen, K.; Groothoff, N.

2005-01-01

A water core photonic crystal Fresnel fiber exploiting a hole distribution on zone plates of a cylindrical waveguide was developed and characterized. This fiber has similar guiding properties as the pristine air-hole guiding fiber although a large loss edge ~900nm is observed indicating that the

Ultrafast laser spectroscopy in complex solid state materials

Energy Technology Data Exchange (ETDEWEB)

Li, Tianqi [Iowa State Univ., Ames, IA (United States)

2014-12-01

This thesis summarizes my work on applying the ultrafast laser spectroscopy to the complex solid state materials. It shows that the ultrafast laser pulse can coherently control the material properties in the femtosecond time scale. And the ultrafast laser spectroscopy can be employed as a dynamical method for revealing the fundamental physical problems in the complex material systems.

Picosecond phase-velocity dispersion of hypersonic phonons imaged with ultrafast electron microscopy

International Nuclear Information System (INIS)

Cremons, Daniel R.; Du, Daniel X.; Flannigan, David J.

2017-01-01

We describe the direct imaging—with four-dimensional ultrafast electron microscopy—of the emergence, evolution, dispersion, and decay of photoexcited, hypersonic coherent acoustic phonons in nanoscale germanium wedges. Coherent strain waves generated via ultrafast in situ photoexcitation were imaged propagating with initial phase velocities of up to 35 km/s across discrete micrometer-scale crystal regions. We then observe that, while each wave front travels at a constant velocity, the entire wave train evolves with a time-varying phase-velocity dispersion, displaying a single-exponential decay to the longitudinal speed of sound (5 km/s) and with a mean lifetime of 280 ps. We also find that the wave trains propagate along a single in-plane direction oriented parallel to striations introduced during specimen preparation, independent of crystallographic direction. Elastic-plate modeling indicates the dynamics arise from excitation of a single, symmetric (dilatational) guided acoustic mode. Further, by precisely determining the experiment time-zero position with a plasma-lensing method, we find that wave-front emergence occurs approximately 100 ps after femtosecond photoexcitation, which matches well with Auger recombination times in germanium. We conclude by discussing the similarities between the imaged hypersonic strain-wave dynamics and electron/hole plasma-wave dynamics in strongly photoexcited semiconductors.

Picosecond phase-velocity dispersion of hypersonic phonons imaged with ultrafast electron microscopy

Science.gov (United States)

Cremons, Daniel R.; Du, Daniel X.; Flannigan, David J.

2017-12-01

Here, we describe the direct imaging—with four-dimensional ultrafast electron microscopy—of the emergence, evolution, dispersion, and decay of photoexcited, hypersonic coherent acoustic phonons in nanoscale germanium wedges. Coherent strain waves generated via ultrafast in situ photoexcitation were imaged propagating with initial phase velocities of up to 35 km/s across discrete micrometer-scale crystal regions. We observe that, while each wave front travels at a constant velocity, the entire wave train evolves with a time-varying phase-velocity dispersion, displaying a single-exponential decay to the longitudinal speed of sound (5 km/s) and with a mean lifetime of 280 ps. We also find that the wave trains propagate along a single in-plane direction oriented parallel to striations introduced during specimen preparation, independent of crystallographic direction. Elastic-plate modeling indicates the dynamics arise from excitation of a single, symmetric (dilatational) guided acoustic mode. Further, by precisely determining the experiment time-zero position with a plasma-lensing method, we find that wave-front emergence occurs approximately 100 ps after femtosecond photoexcitation, which matches well with Auger recombination times in germanium. We conclude by discussing the similarities between the imaged hypersonic strain-wave dynamics and electron/hole plasma-wave dynamics in strongly photoexcited semiconductors.

Ultrafast terahertz electrodynamics of photonic and electronic nanostructures

Energy Technology Data Exchange (ETDEWEB)

Luo, Liang [Iowa State Univ., Ames, IA (United States)

2015-01-01

This thesis summarizes my work on using ultrafast laser pulses to study Terahertz (THz) electrodynamics of photonic and electronic nanostructures and microstructures. Ultrafast timeresolved (optical, NIR, MIR, THz) pump-probe spectroscopy setup has been successfully built, which enables me to perform a series of relevant experiments. Firstly, a novel high e ciency and compact THz wave emitter based on split-ring-resonators has been developed and characterized. The emitter can be pumped at any wavelength by tailoring the magnetic resonance and could generate gapless THz waves covering the entire THz band. Secondly, two kinds of new photonic structures for THz wave manipulation have been successfully designed and characterized. One is based on the 1D and 2D photo-imprinted di ractive elements. The other is based on the photoexcited double-split-ring-resonator metamaterials. Both structures are exible and can modulate THz waves with large tunability. Thirdly, the dark excitons in semiconducting singlewalled carbon nanotubes are studied by optical pump and THz probe spectroscopy, which provides the rst insights into the THz responses of nonequilibrium excitonic correlations and dynamics from the dark ground states in carbon nanotubes. Next, several on-going projects are brie y presented such as the study of ultrafast THz dynamics of Dirac fermions in topological insulator Bi₂Se₃ with Mid-infrared excitation. Finally, the thesis ends with a summary of the completed experiments and an outlook of the future plan.

Temporal reflectance from a light pulse irradiated medium embedded with highly scattering cores

International Nuclear Information System (INIS)

Hsu Peifeng; Lu Xiaodong

2007-01-01

This paper presents a new approach to utilize ultrashort pulsed laser for optical diagnostics with numerical simulations. The method is based on the use of ultrafast pulses with a pulsewidth selected according to the probed medium's radiative property and/or size. Our previous work in nonhomogeneous media has shown that the resulting time-resolved reflectance signal will have a unique characteristic: it will show a direct correlation of ballistic photon travel time and interface location, which is in between different layers or nonhomogeneous regions. The premise is based on utilizing the medium's structural information carried by the ballistic and snake photons without being masked by the diffuse photons. In this study, the space-time correlation is further explored in the case of minimally scattered photons from a large scattering coefficient core region embedded within a less-scattering medium. Time-resolved reflectance signals of the single scattering core and multiple scattering cores within a three-dimensional medium demonstrate the concept and illustrate the additional effect due to the scattered photons from the core region. A unique temporal signal profile's correlation at various detector positions with respect to the scattering core is explained in detail. The result has important implications. This approach will lead to a much simpler and more precise determination of the probed medium's composition or structure. Due to the large computational requirement to obtain the physical details of the light pulse propagation inside highly scattering multi-dimensional media, the reverse Monte-Carlo method is used. The potential applications of the method include non-destructive diagnostics, optical imaging, and remote sensing of underwater objects

Deep-lying hole states in the optical model

International Nuclear Information System (INIS)

Klevansky, S.P.; Lemmer, R.H.

1982-01-01

The strength function for deep-lying hole states in an optical potential is studied by the method of Green's functions. The role of isospin is emphasized. It is shown that, while the main trends of the experimental data on hole states in isotopes of Sn and Pd can be described by an energy independent optical potential, intermediate structures in these data indicate the specific nuclear polarization effects have to be included. This is done by introducing doorway states of good isospin into the optical model potential. Such states consist of neutron hole plus proton core vibrations as well as more complicated excitations that are analog states of proton hole plus neutron core vibrations of the parent nuclear system. Specific calculations for 115 Sn and 103 Pd give satisfactory fits to the strength function data using optical model and doorway state parameters that are reasonable on physical grounds

Do Nuclear Star Clusters and Supermassive Black Holes Follow the Same Host-Galaxy Correlations?

Directory of Open Access Journals (Sweden)

Peter Erwin

2012-01-01

Full Text Available Studies have suggested that there is a strong correlation between the masses of nuclear star clusters (NSCs and their host galaxies, a correlation which is said to be an extension of the well-known correlations between supermassive black holes (SMBHs and their host galaxies. But careful analysis of disk galaxies—including 2D bulge/disk/bar decompositions—shows that while SMBHs correlate with the stellar mass of the bulge component of galaxies, the masses of NSCs correlate much better with the total galaxy stellar mass. In addition, the mass ratio MNSC/M⋆, tot for NSCs in spirals (at least those with Hubble types Sc and later is typically an order of magnitude smaller than the mass ratio MBH/M⋆, bul of SMBHs. The absence of a universal “central massive object” correlation argues against common formation and growth mechanisms for both SMBHs and NSCs. We also discuss evidence for a break in the NSC-host galaxy correlation, galaxies with Hubble types earlier than Sbc appear to host systematically more massive NSCs than do types Sc and later.

Seven Hints for Primordial Black Hole Dark Matter arXiv

CERN Document Server

Clesse, Sebastien

Seven observations point towards the existence of primordial black holes (PBH), constituting the whole or an important fraction of the dark matter in the Universe: the mass and spin of black holes detected by Advanced LIGO/VIRGO, the detection of micro-lensing events of distant quasars and stars in M31, the non-detection of ultra-faint dwarf satellite galaxies with radius below 15 parsecs, evidences for core galactic dark matter profiles, the correlation between X-ray and infrared cosmic backgrounds, and the existence of super-massive black holes very early in the Universe's history. Some of these hints are newly identified and they are all intriguingly compatible with the re-constructed broad PBH mass distribution from LIGO events, peaking on PBH mass $m_{\\rm PBH} \\approx 3 M_\\odot$ and passing all other constraints on PBH abundances. PBH dark matter also provides a new mechanism to explain the mass-to-light ratios of dwarf galaxies, including the recent detection of a diffuse galaxy not dominated by dark ma...

Effect of strong correlations on the high energy anomaly in hole- and electron-doped high-Tc superconductors

International Nuclear Information System (INIS)

Moritz, B; Johnston, S; Greven, M; Shen, Z-X; Devereaux, T P; Schmitt, F; Meevasana, W; Motoyama, E M; Lu, D H; Kim, C; Scalettar, R T

2009-01-01

Recently, angle-resolved photoemission spectroscopy (ARPES) has been used to highlight an anomalously large band renormalization at high binding energies in cuprate superconductors: the high energy 'waterfall' or high energy anomaly (HEA). This paper demonstrates, using a combination of new ARPES measurements and quantum Monte Carlo simulations, that the HEA is not simply the by-product of matrix element effects, but rather represents a cross-over from a quasi-particle band at low binding energies near the Fermi level to valence bands at higher binding energy, assumed to be of strong oxygen character, in both hole- and electron-doped cuprates. While photoemission matrix elements clearly play a role in changing the aesthetic appearance of the band dispersion, i.e. the 'waterfall'-like behavior, they provide an inadequate description for the physics that underlies the strong band renormalization giving rise to the HEA. Model calculations of the single-band Hubbard Hamiltonian showcase the role played by correlations in the formation of the HEA and uncover significant differences in the HEA energy scale for hole- and electron-doped cuprates. In addition, this approach properly captures the transfer of spectral weight accompanying both hole and electron doping in a correlated material and provides a unifying description of the HEA across both sides of the cuprate phase diagram.

Understanding the fate of merging supermassive black holes

International Nuclear Information System (INIS)

Campanelli, Manuela

2005-01-01

Understanding the fate of merging supermassive black holes in galactic mergers, and the gravitational wave emission from this process, are important LISA science goals. To this end, we present results from numerical relativity simulations of binary black hole mergers using the so-called Lazarus approach to model gravitational radiation from these events. In particular, we focus here on some recent calculations of the final spin and recoil velocity of the remnant hole formed at the end of a binary black hole merger process, which may constrain the growth history of massive black holes at the core of galaxies and globular clusters

Support structure for reactor core constituent element

International Nuclear Information System (INIS)

Aida, Yasuhiko.

1993-01-01

A connection pipe having an entrance nozzle inserted therein as a reactor core constituent element is protruded above the upper surface of a reactor core support plate. A through hole is disposed to the protruding portion of the connection pipe. The through hole and a through hole disposed to the reactor core support plate are connected by a communication pipe. A shear rod is disposed in a horizontal portion at the inside of the communication pipe and is supported by a spring horizontally movably. Further, a groove is disposed at a position of the entrance nozzle opposing to the shear rod. The shear rod is urged out of the communication pipe by the pressure of the high pressure plenum and the top end portion of the shear rod is inserted to the groove of the entrance nozzle during operation. Accordingly, the shear rod is positioned in a state where it is extended from the through hole of the communication pipe to the groove of the entrance nozzle. This can mechanically constrain the rising of the reactor core constituent elements by the shear rod upon occurrence of earthquakes. (I.N.)

Real-Time Observation of Ultrafast Intraband Relaxation and Exciton Multiplication in PbS Quantum Dots

KAUST Repository

El-Ballouli, Ala’a O.

2014-03-19

We examine ultrafast intraconduction band relaxation and multiple-exciton generation (MEG) in PbS quantum dots (QDs) using transient absorption spectroscopy with 120 fs temporal resolution. The intraconduction band relaxation can be directly and excellently resolved spectrally and temporally by applying broadband pump-probe spectroscopy to excite and detect the wavelengths around the exciton absorption peak, which is located in the near-infrared region. The time-resolved data unambiguously demonstrate that the intraband relaxation time progressively increases as the pump-photon energy increases. Moreover, the relaxation time becomes much shorter as the size of the QDs decreases, indicating the crucial role of spatial confinement in the intraband relaxation process. Additionally, our results reveal the systematic scaling of the intraband relaxation time with both excess energy above the effective energy band gap and QD size. We also assess MEG in different sizes of the QDs. Under the condition of high-energy photon excitation, which is well above the MEG energy threshold, ultrafast bleach recovery due to the nonradiative Auger recombination of the multiple electron-hole pairs provides conclusive experimental evidence for the presence of MEG. For instance, we achieved quantum efficiencies of 159, 129 and 106% per single-absorbed photon at pump photoexcition of three times the band gap for QDs with band gaps of 880 nm (1.41 eV), 1000 nm (1.24 eV) and 1210 nm (1.0 eV), respectively. These findings demonstrate clearly that the efficiency of transferring excess photon energy to carrier multiplication is significantly increased in smaller QDs compared with larger ones. Finally, we discuss the Auger recombination dynamics of the multiple electron-hole pairs as a function of QD size.

Black hole feedback in a multiphase interstellar medium

Science.gov (United States)

Bourne, Martin A.; Nayakshin, Sergei; Hobbs, Alexander

2014-07-01

Ultrafast outflows (UFOs) from supermassive black holes (SMBHs) are thought to regulate the growth of SMBHs and host galaxies, resulting in a number of observational correlations. We present high-resolution numerical simulations of the impact of a thermalized UFO on the ambient gas in the inner part of the host galaxy. Our results depend strongly on whether the gas is homogeneous or clumpy. In the former case all of the ambient gas is driven outward rapidly as expected based on commonly used energy budget arguments, while in the latter the flows of mass and energy de-couple. Carrying most of the energy, the shocked UFO escapes from the bulge via paths of least resistance, taking with it only the low-density phase of the host. Most of the mass is however in the high-density phase, and is affected by the UFO much less strongly, and may even continue to flow inwards. We suggest that the UFO energy leakage through the pores in the multiphase interstellar medium (ISM) may explain why observed SMBHs are so massive despite their overwhelmingly large energy production rates. The multiphase ISM effects reported here are probably under-resolved in cosmological simulations but may be included in prescriptions for active galactic nuclei feedback in future simulations and in semi-analytical models.

Drilling holes in rock for final storage of spent nuclear fuel

International Nuclear Information System (INIS)

Nord, G.

1980-09-01

This report delas with the technical and economic aspects of the drilling of vertical holes with diameters of 1.5 metres and 1 metre in the Swedish bedrock. The holes will be 7.7 metres in depth and located on a level approximately 500 metres below the ground surface. There is no directly applicable technique for the construction of the above-mentioned holes from a small tunnel. The data presented in this report are based to a great extent on information supplied by the manufacturers of drilling equipment, and by underground construction contractors. Three different techniques for drilling the holes have been delat with in the report: shaft boring, stitch drilling (three alternative methods) and core drilling. In order to produce the required 233 holes per year, the following sets of equipment must be purchased, and personnel engaged. A hole with a diameter of 1.5 m and a depth of 7.7 m requires 3 to 7 sets of equipment for shaft boring or stitch drilling and engages 12 to 27 employees. The cost per hole varies between 24.200 and 31.200 SKr. Core drilling requires 7 sets of equipment, engages 29 persons and costs 55.300 SKr per hole. A hole with a diameter of 1.0 m requires less personnel and costs between 19.700 and 25.800 per hole except for core drilling where the cost per hole is estimated to 43.900 SKr. Interest costs account for 10 percent - 15 percent of the above-mentioned costs. Our aim has been to calculate the costs for the different methods on as similar a basis as possible, but a margin of error of +- 15 percent entails and overlapping of the cost span for most of the methods considered. (G.B.)

NuSTAR Reveals Relativistic Reflection But No Ultra-Fast Outflow in the Quasar Pg∼1211+143

Science.gov (United States)

Zoghbi, A.; Miller, J. M.; Walton, D. J.; Harrison, F. A.; Fabian, A. C.; Reynolds, C. S.; Boggs, S. E.; Christensen, F. E.; Craig, W.; Hailey, C. J.; Stern, D.; Zhang, W. W.

2015-01-01

We report on four epochs of observations of the quasar PG 1211+143 using NuSTAR. The net exposure time is 300 ks. Prior work on this source found suggestive evidence of an ultra-fast outflow (UFO) in the Fe K band with a velocity of approximately 0.1c. The putative flow would carry away a high-mass flux and kinetic power, with broad implications for feedback and black hole--galaxy co-evolution. NuSTAR detects PG 1211+143 out to 30 keV, meaning that the continuum is well-defined both through and above the Fe K band. A characteristic relativistic disk reflection spectrum is clearly revealed via a broad Fe K emission line and Compton back-scattering curvature. The data offer only weak constraints on the spin of the black hole. A careful search for UFOs shows no significant absorption feature above 90% confidence. The limits are particularly tight when relativistic reflection is included. We discuss the statistics and the implications of these results in terms of connections between accretion onto quasars, Seyferts, and stellar-mass black holes, and feedback into their host environments.

NuSTAR REVEALS RELATIVISTIC REFLECTION BUT NO ULTRA-FAST OUTFLOW IN THE QUASAR PG 1211+143

International Nuclear Information System (INIS)

Zoghbi, A.; Miller, J. M.; Walton, D. J.; Stern, D.; Harrison, F. A.; Fabian, A. C.; Reynolds, C. S.; Boggs, S. E.; Craig, W.; Christensen, F. E.; Hailey, C. J.; Zhang, W. W.

2015-01-01

We report on four epochs of observations of the quasar PG 1211+143 using NuSTAR. The net exposure time is 300 ks. Prior work on this source found suggestive evidence of an ultra-fast outflow (UFO) in the Fe K band with a velocity of approximately 0.1c. The putative flow would carry away a high-mass flux and kinetic power, with broad implications for feedback and black hole--galaxy co-evolution. NuSTAR detects PG 1211+143 out to 30 keV, meaning that the continuum is well-defined both through and above the Fe K band. A characteristic relativistic disk reflection spectrum is clearly revealed via a broad Fe K emission line and Compton back-scattering curvature. The data offer only weak constraints on the spin of the black hole. A careful search for UFOs shows no significant absorption feature above 90% confidence. The limits are particularly tight when relativistic reflection is included. We discuss the statistics and the implications of these results in terms of connections between accretion onto quasars, Seyferts, and stellar-mass black holes, and feedback into their host environments

NuSTAR REVEALS RELATIVISTIC REFLECTION BUT NO ULTRA-FAST OUTFLOW IN THE QUASAR PG 1211+143

Energy Technology Data Exchange (ETDEWEB)

Zoghbi, A.; Miller, J. M. [Department of Astronomy, University of Michigan, 1085 South University Avenue, Ann Arbor, MI 48109 (United States); Walton, D. J.; Stern, D. [Jet Propulsion Laboratory, California Institute of Technology, Pasadena, CA 91109 (United States); Harrison, F. A. [Space Radiation Laboratory, California Institute of Technology, Pasadena, CA 91125 (United States); Fabian, A. C. [Institute of Astronomy, University of Cambridge, Madingley Road, Cambridge, CB3 OHA (United Kingdom); Reynolds, C. S. [Department of Astronomy, University of Maryland, College Park, MD 20742-2421 (United States); Boggs, S. E.; Craig, W. [Space Science Laboratory, University of California, Berkeley, CA 94720 (United States); Christensen, F. E. [DTU Space. National Space Institute, Technical University of Denmark, Elektrovej 327, DK-2800 Lyngby (Denmark); Hailey, C. J. [Columbia Astrophysics Laboratory, Columbia University, New York, NY 10027 (United States); Zhang, W. W., E-mail: abzoghbi@umich.edu [NASA Goddard Space Flight Center, Greenbelt, MD 20771 (United States)

2015-02-01

We report on four epochs of observations of the quasar PG 1211+143 using NuSTAR. The net exposure time is 300 ks. Prior work on this source found suggestive evidence of an ultra-fast outflow (UFO) in the Fe K band with a velocity of approximately 0.1c. The putative flow would carry away a high-mass flux and kinetic power, with broad implications for feedback and black hole--galaxy co-evolution. NuSTAR detects PG 1211+143 out to 30 keV, meaning that the continuum is well-defined both through and above the Fe K band. A characteristic relativistic disk reflection spectrum is clearly revealed via a broad Fe K emission line and Compton back-scattering curvature. The data offer only weak constraints on the spin of the black hole. A careful search for UFOs shows no significant absorption feature above 90% confidence. The limits are particularly tight when relativistic reflection is included. We discuss the statistics and the implications of these results in terms of connections between accretion onto quasars, Seyferts, and stellar-mass black holes, and feedback into their host environments.

Preliminary geologic and geophysical data of the UE25a-3 exploratory drill hole, Nevada Test Site, Nevada

International Nuclear Information System (INIS)

Maldonado, F.; Muller, D.C.; Morrison, J.N.

1979-09-01

The UE25a-3 drill hole, located in the Calico Hills area, was drilled as part of an effort to evaluate the Calico Hills area as a possible nuclear waste repository site. The purpose of the drill hole was to verify the existence of an intrusive crystalline body in the subsurface and to determine the stratigraphy, structure, and nature of fractures of the cored rocks. Cored samples were obtained for mineral, chemical, and material property analyses. Numerous high-angle faults and brecciated zones were intersected by the drill hole. The units cored were intensely fractured with fracture analysis of the core consisting of frequency of fractures, dips of fractures, open and closed (sealed) fractures and types of fracture sealing or coating material. Twenty-four hundred and thirty fractures, representing approximately 30 percent of the fractures present, indicate an average fracture frequency of 13.2 fractures per meter, predominantly high-angle dips with 66 percent of the fractures closed. Fractures in the argillite interval are sealed or coated predominantly with kaolinite, nacrite, and dickite. Calcite, chlorite, and magnetite are present in fractures in the altered argillite interval. Fractures in the marble interval are sealed or coated with calcite, dolomite, and ferruginous clay. The core index indicates that the lower half of the drilled interval is more competent than the upper half. Borehole geophysical logs were run by the Birdwell Division of Seismograph Service Corporation for geologic correlations and lithologic characterizations. The logs include: caliper, density, resistivity, spontaneous potential, Vibroseis, 3-D velocity, neutron, and gamma-ray logs

Probing the quantum correlation and Bell non-locality for Dirac particles with Hawking effect in the background of Schwarzschild black hole

International Nuclear Information System (INIS)

Xu, Shuai; Song, Xue-ke; Shi, Jia-dong; Ye, Liu

2014-01-01

In this Letter, we analytically explore the effect of the Hawking radiation on the quantum correlation and Bell non-locality for Dirac particles in the background of Schwarzschild black hole. It is shown that when the Hawking effect is almost nonexistent, corresponding to the case of an almost extreme black hole, the quantum properties of physically accessible state are the same for the initial situation. For finite Hawking temperature T, the accessible quantum correlation monotonously decreases along with increasing T owing to the thermal fields generated by the Hawking effect, and the accessible quantum non-locality will be disappeared when the Hawking temperature is more than a fixed value which increases with the parameter r of Werner state growing. Then we analyze the redistribution of quantum correlation, and find that for the case of the Hawking temperature being infinite, corresponding to the case of the black hole evaporating completely, the quantum correlation of physically accessible state is equal to the one of the inaccessible states. Moreover, due to the Pauli exclusion principle and the differences between Fermi–Dirac and Bose–Einstein statistics, for the Dirac fields the accessible classical correlation decreases with increase of the Hawking temperature, which is different for the scalar fields. For Bell non-locality, we also find that the quantum non-locality is always extinct for physically inaccessible states, and the strength of the non-locality decreases with enlarging intensity of Hawking effect when the non-locality is existent in physically accessible state.

Short-Range Correlated Magnetic Core-Shell CrO₂/Cr₂O₃ Nanorods: Experimental Observations and Theoretical Considerations.

Science.gov (United States)

Gandhi, Ashish C; Li, Tai-Yue; Chan, Ting Shan; Wu, Sheng Yun

2018-05-09

With the evolution of synthesis and the critical characterization of core-shell nanostructures, short-range magnetic correlation is of prime interest in employing their properties to develop novel devices and widespread applications. In this regard, a novel approach of the magnetic core-shell saturated magnetization (CSSM) cylinder model solely based on the contribution of saturated magnetization in one-dimensional CrO₂/Cr₂O₃ core-shell nanorods (NRs) has been developed and applied for the determination of core-diameter and shell-thickness. The nanosized effect leads to a short-range magnetic correlation of ferromagnetic core-CrO₂ extracted from CSSM, which can be explained using finite size scaling method. The outcome of this study is important in terms of utilizing magnetic properties for the critical characterization of core-shell nanomagnetic materials.

Ultrafast Dynamics of Metallo-Dielectric Core-Shell Particles

NARCIS (Netherlands)

Shan, X.

2008-01-01

Optical properties of metallic nano-structures have attracted a lot of attention in the past decades. In this thesis, we focus on nano-sized silica-core gold-shell particles, study the linear, nonlinear and acoustic vibrations of the particles. The linear optical properties in the visible range of

Covariance mapping of two-photon double core hole states in C 2 H 2 and C 2 H 6 produced by an x-ray free electron laser

International Nuclear Information System (INIS)

Mucke, M; Motomura, K; Bozek, J D; Schorb, S; Messerschmidt, M; Glownia, J M; Cryan, J P; Coffee, R N; Takahashi, O; Prince, K C; Feifel, R; Univ. of Gothenburg

2015-01-01

Few-photon ionization and relaxation processes in acetylene (C 2 H 2 ) and ethane (C 2 H 6 ) were investigated at the linac coherent light source x-ray free electron laser (FEL) at SLAC, Stanford using a highly efficient multi-particle correlation spectroscopy technique based on a magnetic bottle. The analysis method of covariance mapping has been applied and enhanced, allowing us to identify electron pairs associated with double core hole (DCH) production and competing multiple ionization processes including Auger decay sequences. The experimental technique and the analysis procedure are discussed in the light of earlier investigations of DCH studies carried out at the same FEL and at third generation synchrotron radiation sources. In particular, we demonstrate the capability of the covariance mapping technique to disentangle the formation of molecular DCH states which is barely feasible with conventional electron spectroscopy methods

Spatial Correlation in the Ambient Core Noise Field of a Turbofan Engine

Science.gov (United States)

Miles, Jeffrey Hilton

2012-01-01

An acoustic transfer function relating combustion noise and turbine exit noise in the presence of enclosed ambient core noise is investigated using a dynamic system model and an acoustic system model for the particular turbofan engine studied and for a range of operating conditions. Measurements of cross-spectra magnitude and phase between the combustor and turbine exit and auto-spectra at the turbine exit and combustor are used to show the presence of indirect and direct combustion noise over the frequency range of 0 400 Hz. The procedure used evaluates the ratio of direct to indirect combustion noise. The procedure used also evaluates the post-combustion residence time in the combustor which is a factor in the formation of thermal NOx and soot in this region. These measurements are masked by the ambient core noise sound field in this frequency range which is observable since the transducers are situated within an acoustic wavelength of one another. An ambient core noise field model based on one and two dimensional spatial correlation functions is used to replicate the spatially correlated response of the pair of transducers. The spatial correlation function increases measured attenuation due to destructive interference and masks the true attenuation of the turbine.

Core-hole-induced dynamical effects in the x-ray emission spectrum of liquid methanol.

Science.gov (United States)

Ljungberg, M P; Zhovtobriukh, I; Takahashi, O; Pettersson, L G M

2017-04-07

We compute the x-ray emission spectrum of liquid methanol, with the dynamical effects that result from the creation of the core hole included in a semiclassical way. Our method closely reproduces a fully quantum mechanical description of the dynamical effects for relevant one-dimensional models of the hydrogen-bonded methanol molecules. For the liquid, we find excellent agreement with the experimental spectrum, including the large isotope effect in the first split peak. The dynamical effects depend sensitively on the initial structure in terms of the local hydrogen-bonding (H-bonding) character: non-donor molecules contribute mainly to the high-energy peak while molecules with a strong donating H-bond contribute to the peak at lower energy. The spectrum thus reflects the initial structure mediated by the dynamical effects that are, however, seen to be crucial in order to reproduce the intensity distribution of the recently measured spectrum.

A novel optical tool for controlling and probing ultrafast surface dynamics

International Nuclear Information System (INIS)

Yang, Yudong

2017-12-01

Ultrashort pulse laser sources have been greatly developed over the past few decades. The available pulse duration has been reduced to the single-cycle pulse regime. The discovery of high harmonic generation has freed us from the limitation of the laser wavelength. Moreover, the demonstration of isolated attosecond pulse generation has indicated the advent of the attosecond science era. Attosecond pulses undoubtedly allow one to study ultrafast dynamics with unprecedented time resolution. However, physical systems with genuine attosecond time scale dynamics are rather challenging to find. Ultrafast surface charge transfer, which is an important process in photochemistry and electrochemistry, is a good candidate experimental system exhibiting attosecond electronic dynamics. Specifically, the ultrafast surface charge transfer on the c(4 x 2)S/Ru(0001) surface was previously studied and the charge transfer time inferred to be 320 as using core-hole clock spectroscopy at a synchrotron facility. In order to measure this benchmark attosecond electronic dynamics with real time-resolving methods, pump pulses centered at 160 eV and probe pulses centered at 40 eV are required. To this end, a dedicated attosecond experimental beamline including an ultrashort laser pulse source and an attosecond pulse generation and characterization setup has been designed and is being developed. The author of this thesis was responsible for the construction of the attosecond experimental beamline which will be used ultrafast surface charge transfer studies. In this thesis, a completely functional attosecond extreme ultraviolet (XUV) beamline, which includes a few-cycle laser pulse source, an attosecond pulse generation and characterization setup, is described. A commercial Ti:sapphire-based chirped-pulse amplification (CPA) laser system is the overall source of the beamline. The laser system is actively carrier-envelope phase (CEP) stabilized and the output pulse duration is ∝35 fs. The

A novel optical tool for controlling and probing ultrafast surface dynamics

Energy Technology Data Exchange (ETDEWEB)

Yang, Yudong

2017-12-15

Ultrashort pulse laser sources have been greatly developed over the past few decades. The available pulse duration has been reduced to the single-cycle pulse regime. The discovery of high harmonic generation has freed us from the limitation of the laser wavelength. Moreover, the demonstration of isolated attosecond pulse generation has indicated the advent of the attosecond science era. Attosecond pulses undoubtedly allow one to study ultrafast dynamics with unprecedented time resolution. However, physical systems with genuine attosecond time scale dynamics are rather challenging to find. Ultrafast surface charge transfer, which is an important process in photochemistry and electrochemistry, is a good candidate experimental system exhibiting attosecond electronic dynamics. Specifically, the ultrafast surface charge transfer on the c(4 x 2)S/Ru(0001) surface was previously studied and the charge transfer time inferred to be 320 as using core-hole clock spectroscopy at a synchrotron facility. In order to measure this benchmark attosecond electronic dynamics with real time-resolving methods, pump pulses centered at 160 eV and probe pulses centered at 40 eV are required. To this end, a dedicated attosecond experimental beamline including an ultrashort laser pulse source and an attosecond pulse generation and characterization setup has been designed and is being developed. The author of this thesis was responsible for the construction of the attosecond experimental beamline which will be used ultrafast surface charge transfer studies. In this thesis, a completely functional attosecond extreme ultraviolet (XUV) beamline, which includes a few-cycle laser pulse source, an attosecond pulse generation and characterization setup, is described. A commercial Ti:sapphire-based chirped-pulse amplification (CPA) laser system is the overall source of the beamline. The laser system is actively carrier-envelope phase (CEP) stabilized and the output pulse duration is ∝35 fs. The

Density matrix-based time-dependent configuration interaction approach to ultrafast spin-flip dynamics

Science.gov (United States)

Wang, Huihui; Bokarev, Sergey I.; Aziz, Saadullah G.; Kühn, Oliver

2017-08-01

Recent developments in attosecond spectroscopy yield access to the correlated motion of electrons on their intrinsic timescales. Spin-flip dynamics is usually considered in the context of valence electronic states, where spin-orbit coupling is weak and processes related to the electron spin are usually driven by nuclear motion. However, for core-excited states, where the core-hole has a nonzero angular momentum, spin-orbit coupling is strong enough to drive spin-flips on a much shorter timescale. Using density matrix-based time-dependent restricted active space configuration interaction including spin-orbit coupling, we address an unprecedentedly short spin-crossover for the example of L-edge (2p→3d) excited states of a prototypical Fe(II) complex. This process occurs on a timescale, which is faster than that of Auger decay (∼4 fs) treated here explicitly. Modest variations of carrier frequency and pulse duration can lead to substantial changes in the spin-state yield, suggesting its control by soft X-ray light.

Middleweight black holes found at last

Science.gov (United States)

Clery, Daniel

2018-06-01

How did giant black holes grow so big? Astronomers have long had evidence of baby black holes with masses of no more than tens of suns, and of million- or billion-solar-mass behemoths lurking at the centers of galaxies. But middle-size ones, weighing thousands or tens of thousands of suns, seemed to be missing. Their absence forced theorists to propose that supermassive black holes didn't grow gradually by slowly consuming matter, but somehow emerged as ready-made giants. Now, astronomers appear to have located some missing middleweights. An international team has scoured an archive of galaxy spectra and found more than 300 small galaxies that have the signature of intermediate mass black holes in their cores, opening new questions for theorists.

Ultrafast surface carrier dynamics in the topological insulator Bi₂Te₃.

Science.gov (United States)

Hajlaoui, M; Papalazarou, E; Mauchain, J; Lantz, G; Moisan, N; Boschetto, D; Jiang, Z; Miotkowski, I; Chen, Y P; Taleb-Ibrahimi, A; Perfetti, L; Marsi, M

2012-07-11

We discuss the ultrafast evolution of the surface electronic structure of the topological insulator Bi(2)Te(3) following a femtosecond laser excitation. Using time and angle-resolved photoelectron spectroscopy, we provide a direct real-time visualization of the transient carrier population of both the surface states and the bulk conduction band. We find that the thermalization of the surface states is initially determined by interband scattering from the bulk conduction band, lasting for about 0.5 ps; subsequently, few picoseconds are necessary for the Dirac cone nonequilibrium electrons to recover a Fermi-Dirac distribution, while their relaxation extends over more than 10 ps. The surface sensitivity of our measurements makes it possible to estimate the range of the bulk-surface interband scattering channel, indicating that the process is effective over a distance of 5 nm or less. This establishes a correlation between the nanoscale thickness of the bulk charge reservoir and the evolution of the ultrafast carrier dynamics in the surface Dirac cone.

Using a Semiconductor-to-Metal Transition to Control Optical Transmission through Subwavelength Hole Arrays

Directory of Open Access Journals (Sweden)

E. U. Donev

2008-01-01

Full Text Available We describe a simple configuration in which the extraordinary optical transmission effect through subwavelength hole arrays in noble-metal films can be switched by the semiconductor-to-metal transition in an underlying thin film of vanadium dioxide. In these experiments, the transition is brought about by thermal heating of the bilayer film. The surprising reverse hysteretic behavior of the transmission through the subwavelength holes in the vanadium oxide suggest that this modulation is accomplished by a dielectric-matching condition rather than plasmon coupling through the bilayer film. The results of this switching, including the wavelength dependence, are qualitatively reproduced by a transfer matrix model. The prospects for effecting a similar modulation on a much faster time scale by using ultrafast laser pulses to trigger the semiconductor-to-metal transition are also discussed.

THE LANDSCAPE OF THE NEUTRINO MECHANISM OF CORE-COLLAPSE SUPERNOVAE: NEUTRON STAR AND BLACK HOLE MASS FUNCTIONS, EXPLOSION ENERGIES, AND NICKEL YIELDS

International Nuclear Information System (INIS)

Pejcha, Ondřej; Thompson, Todd A.

2015-01-01

If the neutrino luminosity from the proto-neutron star formed during a massive star core collapse exceeds a critical threshold, a supernova (SN) results. Using spherical quasi-static evolutionary sequences for hundreds of progenitors over a range of metallicities, we study how the explosion threshold maps onto observables, including the fraction of successful explosions, the neutron star (NS) and black hole (BH) mass functions, the explosion energies (E SN ) and nickel yields (M Ni ), and their mutual correlations. Successful explosions are intertwined with failures in a complex pattern that is not simply related to initial progenitor mass or compactness. We predict that progenitors with initial masses of 15 ± 1, 19 ± 1, and ∼21-26 M ☉ are most likely to form BHs, that the BH formation probability is non-zero at solar-metallicity and increases significantly at low metallicity, and that low luminosity, low Ni-yield SNe come from progenitors close to success/failure interfaces. We qualitatively reproduce the observed E SN -M Ni correlation, we predict a correlation between the mean and width of the NS mass and E SN distributions, and that the means of the NS and BH mass distributions are correlated. We show that the observed mean NS mass of ≅ 1.33 M ☉ implies that the successful explosion fraction is higher than 0.35. Overall, we show that the neutrino mechanism can in principle explain the observed properties of SNe and their compact objects. We argue that the rugged landscape of progenitors and outcomes mandates that SN theory should focus on reproducing the wide ranging distributions of observed SN properties

Measuring proton shift tensors with ultrafast MAS NMR.

Science.gov (United States)

Miah, Habeeba K; Bennett, David A; Iuga, Dinu; Titman, Jeremy J

2013-10-01

A new proton anisotropic-isotropic shift correlation experiment is described which operates with ultrafast MAS, resulting in good resolution of isotropic proton shifts in the detection dimension. The new experiment makes use of a recoupling sequence designed using symmetry principles which reintroduces the proton chemical shift anisotropy in the indirect dimension. The experiment has been used to measure the proton shift tensor parameters for the OH hydrogen-bonded protons in tyrosine·HCl and citric acid at Larmor frequencies of up to 850 MHz. Copyright © 2013 Elsevier Inc. All rights reserved.

Black Hole Safari: Tracking Populations and Hunting Big Game

Science.gov (United States)

McConnell, N. J.

2013-10-01

Understanding the physical connection, or lack thereof, between the growth of galaxies and supermassive black holes is a key challenge in extragalactic astronomy. Dynamical studies of nearby galaxies are building a census of black hole masses across a broad range of galaxy types and uncovering statistical correlations between galaxy bulge properties and black hole masses. These local correlations provide a baseline for studying galaxies and black holes at higher redshifts. Recent measurements have probed the extremes of the supermassive black hole population and introduced surprises that challenge simple models of black hole and galaxy co-evolution. Future advances in the quality and quantity of dynamical black hole mass measurements will shed light upon the growth of massive galaxies and black holes in different cosmic environments.

Site selective dissociation of ozone upon core excitation

International Nuclear Information System (INIS)

Mocellin, A.; Mundim, M.S.P.; Coutinho, L.H.; Homem, M.G.P.; Naves de Brito, A.

2007-01-01

We present new measurements applied to core excitation of ozone molecule using to analyze the dissociation channels the photo-electron-photo-ion coincidence (PEPICO) and the photo-electron-photo-ion-photo-ion coincidence (PEPIPICO) technique. The new experimental set-up allows measuring O + /O + ion pair coincidences without discrimination. The dissociation channels of several core-excited states have been investigated. The relative yields of dissociation channels were determined from coincidence data. The core excitation from O terminal (O T ) or O central (O C ) induce different fragmentation; preferentially one bond is broken at the O terminal excitation and two bonds when O central is excited, showing site selectivity fragmentation of ozone upon core excitation. The ultra-fast dissociation of the O T 1s -1 7a 1 1 core-excited state is confirmed by the relative yield of dissociation

Identification of Columbia River basalt flows from deep cores in the Pasco Basin based on trace element abundances

International Nuclear Information System (INIS)

Fruchter, J.S.; Rancitelli, L.A.

1976-01-01

Samples of basalt from three deep core holes drilled in the Pasco Basin, Washington (DDH-3, DH-4, DH-5) were analyzed by instrumental neutron activation (INAA) for up to fifteen trace and major elements. These analyses were used to assign each basalt flow to one of a series of previously defined chemical types of the Columbia River Basalt Group. All of the flows except the two flows at the bottom of well DDH-3 were clearly assignable to one of the defined chemical types. These two flows apparently represent new, as yet undefined chemical types. Average values and standard deviations for compositions of each of the chemical types found in the three wells are presented along with two-element variation diagrams for the geochemically important pair La-Cr, La-Fe, La-Th and La-Sc. The assignment of the flows to known chemical types accomplished in this study was very helpful in relating the basalts in the core holes to stratigraphically defined basalt flows in surface sections. A correlation diagram relating the flows in the core holes to one another on the basis of chemical type is presented

Relativistic three-body effects in black hole coalescence

International Nuclear Information System (INIS)

Campanelli, Manuela; Dettwyler, Miranda; Lousto, Carlos O.; Hannam, Mark

2006-01-01

Three-body interactions are expected to be common in globular clusters and in galactic cores hosting supermassive black holes. We consider an equal-mass binary black hole system in the presence of a third black hole. Using numerically generated binary black hole initial data sets, and first and second-order post-Newtonian (1PN and 2PN) techniques, we find that the presence of the third black hole has non-negligible relativistic effects on the location of the binary's innermost stable circular orbit (ISCO), and that these effects arise at 2PN order. For a stellar-mass black hole binary in orbit about a supermassive black hole, the massive black hole has stabilizing effects on the orbiting binary, leading to an increase in merger time and a decrease of the terminal orbital frequency, and an amplification of the gravitational radiation emitted from the binary system by up to 6%

Data for four geologic test holes in the Sacramento Valley, California

Science.gov (United States)

Berkstresser, C.F.; French, J.J.; Schaal, M.E.

1985-01-01

The report provides geological and geophysical data for four of seven test holes drilled as a part of the Central Valley Aquifer Project, which is part of the Regional Aquifer Systems Analysis. The holes were drilled with a rotary well drilling machine to depths of 900 feet in the southwestern part of the Sacramento Valley in Solano and Yolo Counties. Geologic data for each well include lithology, texture, color, character of the contact, sorting, rounding, and cementation, determined from cuttings, cores, and sidewall covers. Fifty cores, 3 feet long, were obtained from each hole, and from eight to fourteen sidewall cores were collected. Geophysical data include a dual-induction log, spherically focused log (SFL), compensated neutron-formation density log, gamma-ray log, and a caliper log. These data are presented in four tables and on four plates. (USGS)

The Cosmogony of Super-Massive Black Holes

International Nuclear Information System (INIS)

Duschl, Wolfgang J; Strittmatter, Peter A

2012-01-01

We summarize our recent results on the evolution of super-massive black holes in the cores of galaxies. Our models are based on the viscous, Eddington-limited evolution of self-gravitating accretion disks. We find that, within this framework, one can explain the growth time scales and the luminosities of individual objects as well as the variation of these quantities for AGN with different black hole masses.

Ultrafast photocurrents and terahertz radiation in gallium arsenide and carbon based nanostructures

Energy Technology Data Exchange (ETDEWEB)

Prechtel, Hans Leonhard

2011-08-15

In this thesis we developed a measurement technique based on a common pump-probe scheme and coplanar stripline circuits that enables time-resolved photocurrent measurements of contacted nanosystems with a micrometer spatial and a picosecond time resolution. The measurement technique was applied to lowtemperature grown gallium arsenide (LT-GaAs), carbon nanotubes (CNTs), graphene, and p-doped gallium arsenide (GaAs) nanowires. The various mechanisms responsible for the generation of current pulses by pulsed laser excitation were reviewed. Furthermore the propagation of the resulting electromagnetic radiation along a coplanar stripline circuit was theoretically and numerically treated. The ultrafast photocurrent response of low-temperature grown GaAs was investigated. We found two photocurrent pulses in the time-resolved response. We showed that the first pulse is consistent with a displacement current pulse. We interpreted the second pulse to result from a transport current process. We further determined the velocity of the photo-generated charge carriers to exceed the drift, thermal and quantum velocities of single charge carriers. Hereby, we interpreted the transport current pulse to stem from an electron-hole plasma excitation. We demonstrated that the photocurrent response of CNTs comprises an ultrafast displacement current and a transport current. The data suggested that the photocurrent is finally terminated by the recombination lifetime of the charge carriers. To the best of our knowledge, we presented in this thesis the first recombination lifetime measurements of contacted, suspended, CVD grown CNT networks. In addition, we studied the ultrafast photocurrent dynamics of freely suspended graphene contacted by metal electrodes. At the graphene-metal interface, we demonstrated that built-in electric fields give rise to a photocurrent with a full-width-half-maximum of a few picoseconds and that a photo-thermoelectric effect generates a current with a decay time

Progress in ultrafast laser processing and future prospects

Science.gov (United States)

Sugioka, Koji

2017-03-01

The unique characteristics of ultrafast lasers have rapidly revolutionized materials processing after their first demonstration in 1987. The ultrashort pulse width of the laser suppresses heat diffusion to the surroundings of the processed region, which minimizes the formation of a heat-affected zone and thereby enables ultrahigh precision micro- and nanofabrication of various materials. In addition, the extremely high peak intensity can induce nonlinear multiphoton absorption, which extends the diversity of materials that can be processed to transparent materials such as glass. Nonlinear multiphoton absorption enables three-dimensional (3D) micro- and nanofabrication by irradiation with tightly focused femtosecond laser pulses inside transparent materials. Thus, ultrafast lasers are currently widely used for both fundamental research and practical applications. This review presents progress in ultrafast laser processing, including micromachining, surface micro- and nanostructuring, nanoablation, and 3D and volume processing. Advanced technologies that promise to enhance the performance of ultrafast laser processing, such as hybrid additive and subtractive processing, and shaped beam processing are discussed. Commercial and industrial applications of ultrafast laser processing are also introduced. Finally, future prospects of the technology are given with a summary.

Spirobifluorene Core-Based Novel Hole Transporting Materials for Red Phosphorescence OLEDs

Directory of Open Access Journals (Sweden)

Ramanaskanda Braveenth

2017-03-01

Full Text Available Two new hole transporting materials, named HTM 1A and HTM 1B, were designed and synthesized in significant yields using the well-known Buchwald Hartwig and Suzuki cross- coupling reactions. Both materials showed higher decomposition temperatures (over 450 °C at 5% weight reduction and HTM 1B exhibited a higher glass transition temperature of 180 °C. Red phosphorescence-based OLED devices were fabricated to analyze the device performances compared to Spiro-NPB and NPB as reference hole transporting materials. Devices consist of hole transporting material as HTM 1B showed better maximum current and power efficiencies of 16.16 cd/A and 11.17 lm/W, at the same time it revealed an improved external quantum efficiency of 13.64%. This efficiency is considerably higher than that of Spiro-NPB and NPB-based reference devices.

Perspective: Ultrafast magnetism and THz spintronics

Energy Technology Data Exchange (ETDEWEB)

Walowski, Jakob; Münzenberg, Markus [Institut für Physik, Ernst-Moritz-Arndt-Universität Greifswald, 17489 Greifswald (Germany)

2016-10-14

This year the discovery of femtosecond demagnetization by laser pulses is 20 years old. For the first time, this milestone work by Bigot and coworkers gave insight directly into the time scales of microscopic interactions that connect the spin and electron system. While intense discussions in the field were fueled by the complexity of the processes in the past, it now became evident that it is a puzzle of many different parts. Rather than providing an overview that has been presented in previous reviews on ultrafast processes in ferromagnets, this perspective will show that with our current depth of knowledge the first applications are developed: THz spintronics and all-optical spin manipulation are becoming more and more feasible. The aim of this perspective is to point out where we can connect the different puzzle pieces of understanding gathered over 20 years to develop novel applications. Based on many observations in a large number of experiments. Differences in the theoretical models arise from the localized and delocalized nature of ferromagnetism. Transport effects are intrinsically non-local in spintronic devices and at interfaces. We review the need for multiscale modeling to address the processes starting from electronic excitation of the spin system on the picometer length scale and sub-femtosecond time scale, to spin wave generation, and towards the modeling of ultrafast phase transitions that altogether determine the response time of the ferromagnetic system. Today, our current understanding gives rise to the first usage of ultrafast spin physics for ultrafast magnetism control: THz spintronic devices. This makes the field of ultrafast spin-dynamics an emerging topic open for many researchers right now.

Perspective: Ultrafast magnetism and THz spintronics

International Nuclear Information System (INIS)

Walowski, Jakob; Münzenberg, Markus

2016-01-01

This year the discovery of femtosecond demagnetization by laser pulses is 20 years old. For the first time, this milestone work by Bigot and coworkers gave insight directly into the time scales of microscopic interactions that connect the spin and electron system. While intense discussions in the field were fueled by the complexity of the processes in the past, it now became evident that it is a puzzle of many different parts. Rather than providing an overview that has been presented in previous reviews on ultrafast processes in ferromagnets, this perspective will show that with our current depth of knowledge the first applications are developed: THz spintronics and all-optical spin manipulation are becoming more and more feasible. The aim of this perspective is to point out where we can connect the different puzzle pieces of understanding gathered over 20 years to develop novel applications. Based on many observations in a large number of experiments. Differences in the theoretical models arise from the localized and delocalized nature of ferromagnetism. Transport effects are intrinsically non-local in spintronic devices and at interfaces. We review the need for multiscale modeling to address the processes starting from electronic excitation of the spin system on the picometer length scale and sub-femtosecond time scale, to spin wave generation, and towards the modeling of ultrafast phase transitions that altogether determine the response time of the ferromagnetic system. Today, our current understanding gives rise to the first usage of ultrafast spin physics for ultrafast magnetism control: THz spintronic devices. This makes the field of ultrafast spin-dynamics an emerging topic open for many researchers right now.

Applications of core level spectroscopy to adsorbates

International Nuclear Information System (INIS)

Nilsson, Anders

2002-01-01

In the following review different applications of core-level spectroscopy to atomic and molecular adsorbates will be shown. Core-holes are created through core-level ionization and X-ray absorption processes and the core-hole decays by radiant and non-radiant processes. This forms the basis for X-ray photoelectron spectroscopy, X-ray absorption spectroscopy, Auger electron spectroscopy and X-ray emission spectroscopy. We will demonstrate how we can use the different methods to obtain information about the chemical state, local geometric structure, nature of chemical bonding and dynamics in electron transfer processes. The adsorption of N 2 and CO on Ni(100) will be used as prototype systems for chemisorption while N 2 on graphite and Ar on Pt for physisorption

Electronic structure and intersubband magnetoabsorption spectra of CdSe/CdS core-shell nanowires

Science.gov (United States)

Xiong, Wen

2016-10-01

The electronic structures of CdSe/CdS core-shell nanowires are calculated based on the effective-mass theory, and it is found that the hole states in CdSe/CdS core-shell nanowires are strongly mixed, which are very different from the hole states in CdSe or CdS nanowires. In addition, we find the three highest hole states at the Γ point are almost localized in the CdSe core and the energies of the hole states in CdSe/CdS core-shell nanowires can be enhanced greatly when the core radius Rc increases and the total radius R is fixed. The degenerate hole states are split by the magnetic field, and the split energies will increase when |Jh | increases from 1/2 to 7/2, while they are almost not influenced by the change of the core radius Rc. The absorption spectra of CdSe/CdS core-shell nanowires at the Γ point are also studied in the magnetic field when the temperature T is considered, and we find there are only two peaks will arise if the core radius Rc and the temperature T increase. The intensity of each optical absorption can be considerably enhanced by increasing the core radius Rc when the temperature T is fixed, it is due to the increase of their optical transition matrix element. Meanwhile, the intensity of each optical absorption can be decreased when the temperature T increases and the core radius Rc is fixed, and this is because the Fermi-Dirac distribution function of the corresponding hole states will increase as the increase of the temperature T.

Planet traps and planetary cores: origins of the planet-metallicity correlation

Energy Technology Data Exchange (ETDEWEB)

Hasegawa, Yasuhiro [Institute of Astronomy and Astrophysics, Academia Sinica (ASIAA), P.O. Box 23-141, Taipei 10641, Taiwan (China); Pudritz, Ralph E., E-mail: yasu@asiaa.sinica.edu.tw, E-mail: pudritz@physics.mcmaster.ca [Department of Physics and Astronomy, McMaster University, Hamilton, ON L8S 4M1 (Canada)

2014-10-10

Massive exoplanets are observed preferentially around high metallicity ([Fe/H]) stars while low-mass exoplanets do not show such an effect. This so-called planet-metallicity correlation generally favors the idea that most observed gas giants at r < 10 AU are formed via a core accretion process. We investigate the origin of this phenomenon using a semi-analytical model, wherein the standard core accretion takes place at planet traps in protostellar disks where rapid type I migrators are halted. We focus on the three major exoplanetary populations—hot Jupiters, exo-Jupiters located at r ≅ 1 AU, and the low-mass planets. We show using a statistical approach that the planet-metallicity correlations are well reproduced in these models. We find that there are specific transition metallicities with values [Fe/H] = –0.2 to –0.4, below which the low-mass population dominates, and above which the Jovian populations take over. The exo-Jupiters significantly exceed the hot Jupiter population at all observed metallicities. The low-mass planets formed via the core accretion are insensitive to metallicity, which may account for a large fraction of the observed super-Earths and hot-Neptunes. Finally, a controlling factor in building massive planets is the critical mass of planetary cores (M {sub c,} {sub crit}) that regulates the onset of rapid gas accretion. Assuming the current data is roughly complete at [Fe/H] > –0.6, our models predict that the most likely value of the 'mean' critical core mass of Jovian planets is (M {sub c,} {sub crit}) ≅ 5 M {sub ⊕} rather than 10 M {sub ⊕}. This implies that grain opacities in accreting envelopes should be reduced in order to lower M {sub c,} {sub crit}.

Three-particle one-hole multiple scattering contribution to the nuclear effective interaction in mass-18 nuclei

International Nuclear Information System (INIS)

Bando, H.; Krenciglowa, E.M.; Ando, K.

1979-01-01

Within the systematic framework of the double partition approach, the three-particle one-hole multiple scattering and Q-box formalisms are combined to give the valence-linked and connected energy-independent effective interaction. All low-lying [2p+3p1h] contributions to the mass-18 effective interaction are evaluated using an essentially exact energy-dependent reaction matrix based on the Reid SC potential. The low-lying one-body field of the core nucleus is treated consistently with the underlying reaction matrix G through particle- and hole-line self-energy insertions. Center-of-mass motion, folded diagrams and starting energy dependence are properly taken into account throughout. The low-lying [2p+3p1h] correlations are strongly damped by self-energy insertions. By incorporating only the folded diagram contributions with origins in the low-lying space, the net effect of all low-lying [2p+3p1h] correlations is to give back the bare-G plus second-order core-polarization spectra which are found to be in respectable agreement with the experimental spectra. However, including the full folded diagram contribution, which has additional contributions from the high-lying space through the energy dependence of G, leads to final spectra which deviate sizably from experiment. The present results are conclusive in the sense that the treatment is essentially exact for low-lying [2p+3p1h] correlations which originate from the high-lying two-particle correlations through the reaction matrix G. (Auth.)

Meltdown reactor core cooling facility

International Nuclear Information System (INIS)

Matsuoka, Tsuyoshi.

1992-01-01

The meltdown reactor core cooling facility comprises a meltdown reactor core cooling tank, a cooling water storage tank situates at a position higher than the meltdown reactor core cooling tank, an upper pipeline connecting the upper portions of the both of the tanks and a lower pipeline connecting the lower portions of them. Upon occurrence of reactor core meltdown, a high temperature meltdown reactor core is dropped on the cooling tank to partially melt the tank and form a hole, from which cooling water is flown out. Since the water source of the cooling water is the cooling water storage tank, a great amount of cooling water is further dropped and supplied and the reactor core is submerged and cooled by natural convection for a long period of time. Further, when the lump of the meltdown reactor core is small and the perforated hole of the meltdown reactor cooling tank is small, cooling water is boiled by the high temperature lump intruding into the meltdown reactor core cooling tank and blown out from the upper pipeline to the cooling water storage tank to supply cooling water from the lower pipeline to the meltdown reactor core cooling tank. Since it is constituted only with simple static facilities, the facility can be simplified to attain improvement of reliability. (N.H.)

Site selective dissociation of ozone upon core excitation

Energy Technology Data Exchange (ETDEWEB)

Mocellin, A. [Instituto de Fisica, Universidade de Brasilia-UnB, Box 04455, CEP 70919-970, Brasilia-DF (Brazil)], E-mail: mocellin@fis.unb.br; Mundim, M.S.P. [Instituto de Fisica, Universidade de Brasilia-UnB, Box 04455, CEP 70919-970, Brasilia-DF (Brazil); Coutinho, L.H. [Instituto de Quimica, Universidade Federal do Rio de Janeiro-UFRJ, Box 68563, CEP 21945-970, Rio de Janeiro-RJ (Brazil); Homem, M.G.P. [Laboratorio Nacional de Luz Sincrotron-LNLS, Box 6192, CEP 13084-971, Campinas-SP (Brazil); Naves de Brito, A. [Laboratorio Nacional de Luz Sincrotron-LNLS, Box 6192, CEP 13084-971, Campinas-SP (Brazil); Instituto de Fisica, Universidade de Brasilia-UnB, Box 04455, CEP 70919-970, Brasilia-DF (Brazil)

2007-05-15

We present new measurements applied to core excitation of ozone molecule using to analyze the dissociation channels the photo-electron-photo-ion coincidence (PEPICO) and the photo-electron-photo-ion-photo-ion coincidence (PEPIPICO) technique. The new experimental set-up allows measuring O{sup +}/O{sup +} ion pair coincidences without discrimination. The dissociation channels of several core-excited states have been investigated. The relative yields of dissociation channels were determined from coincidence data. The core excitation from O terminal (O{sub T}) or O central (O{sub C}) induce different fragmentation; preferentially one bond is broken at the O terminal excitation and two bonds when O central is excited, showing site selectivity fragmentation of ozone upon core excitation. The ultra-fast dissociation of the O{sub T} 1s{sup -1}7a{sub 1}{sup 1} core-excited state is confirmed by the relative yield of dissociation.

Slim hole drilling and testing strategies

Science.gov (United States)

Nielson, Dennis L.; Garg, Sabodh K.; Goranson, Colin

2017-12-01

The financial and geologic advantages of drilling slim holes instead of large production wells in the early stages of geothermal reservoir assessment has been understood for many years. However, the practice has not been fully embraced by geothermal developers. We believe that the reason for this is that there is a poor understanding of testing and reservoir analysis that can be conducted in slim holes. In addition to reservoir engineering information, coring through the cap rock and into the reservoir provides important data for designing subsequent production well drilling and completion. Core drilling requires significantly less mud volume than conventional rotary drilling, and it is typically not necessary to cure lost circulation zones (LCZ). LCZs should be tested by either production or injection methods as they are encountered. The testing methodologies are similar to those conducted on large-diameter wells; although produced and/or injected fluid volumes are much less. Pressure, temperature and spinner (PTS) surveys in slim holes under static conditions can used to characterize temperature and pressure distribution in the geothermal reservoir. In many cases it is possible to discharge slim holes and obtain fluid samples to delineate the geochemical properties of the reservoir fluid. Also in the latter case, drawdown and buildup data obtained using a downhole pressure tool can be employed to determine formation transmissivity and well properties. Even if it proves difficult to discharge a slim hole, an injection test can be performed to obtain formation transmissivity. Given the discharge (or injection) data from a slimhole, discharge properties of a large-diameter well can be inferred using wellbore modeling. Finally, slim hole data (pressure, temperature, transmissivity, fluid properties) together with reservoir simulation can help predict the ability of the geothermal reservoir to sustain power production.

Refractive Index Sensor Using a Two-Hole Fiber

Energy Technology Data Exchange (ETDEWEB)

Lopez-Cortes, D; Sanchez-Mondragon, J J [Photonics and Optical Physics Laboratory, Optics Department, INAOE Apdo. Postal 51 and 216, Tonantzintla, Puebla 72000 (Mexico); Margulis, W [Department Fiber Photonics, ACREO, Electrum 236, 16440 Stockholm (Sweden); Dominguez-Cruz, R; May-Arrioja, D A, E-mail: darrioja@uat.edu.mx [Depto. de Ingenieria Electronica, UAM Reynosa Rodhe, Universidad Autonoma de Tamaulipas, Carr. Reynosa-San Fernando S/N, Reynosa, Tamaulipas 88779 (Mexico)

2011-01-01

We propose to use a twin-hole fiber to measure refractive index of liquids. The key idea is to have a single mode fiber (SMF) having two large air-holes running along the fiber length, the holes do not interact with the core. However, using wet chemical etching we can have access to the hole around the fiber, and further etching increases the holes diameter. The diameter is increased until the fiber exhibits a specific birefringence. Since the holes are open, by immersing the fiber in different liquids (n=1.33 to n=1.42) the value of the birefringence is modified and the refractive index of the liquid can be estimated from the change on the beat length. This process provides a very simple and highly sensitive mechanism for sensing refractive index in liquids, and can also be used for other applications.

Photoinduced molecular chirality probed by ultrafast resonant X-ray spectroscopy

Directory of Open Access Journals (Sweden)

Jérémy R. Rouxel

2017-07-01

Full Text Available Recently developed circularly polarized X-ray light sources can probe the ultrafast chiral electronic and nuclear dynamics through spatially localized resonant core transitions. We present simulations of time-resolved circular dichroism signals given by the difference of left and right circularly polarized X-ray probe transmission following an excitation by a circularly polarized optical pump with the variable time delay. Application is made to formamide which is achiral in the ground state and assumes two chiral geometries upon optical excitation to the first valence excited state. Probes resonant with various K-edges (C, N, and O provide different local windows onto the parity breaking geometry change thus revealing the enantiomer asymmetry.

THE TIDAL DISRUPTION OF GIANT STARS AND THEIR CONTRIBUTION TO THE FLARING SUPERMASSIVE BLACK HOLE POPULATION

International Nuclear Information System (INIS)

MacLeod, Morgan; Guillochon, James; Ramirez-Ruiz, Enrico

2012-01-01

Sun-like stars are thought to be regularly disrupted by supermassive black holes (SMBHs) within galactic nuclei. Yet, as stars evolve off the main sequence their vulnerability to tidal disruption increases drastically as they develop a bifurcated structure consisting of a dense core and a tenuous envelope. Here we present the first hydrodynamic simulations of the tidal disruption of giant stars and show that the core has a substantial influence on the star's ability to survive the encounter. Stars with more massive cores retain large fractions of their envelope mass, even in deep encounters. Accretion flares resulting from the disruption of giant stars should last for tens to hundreds of years. Their characteristic signature in transient searches would not be the t –5/3 decay typically associated with tidal disruption events, but a correlated rise over many orders of magnitude in brightness on timescales of months to years. We calculate the relative disruption rates of stars of varying evolutionary stages in typical galactic centers, then use our results to produce Monte Carlo realizations of the expected flaring event populations. We find that the demographics of tidal disruption flares are strongly dependent on both stellar and black hole mass, especially near the limiting SMBH mass scale of ∼10 8 M ☉ . At this black hole mass, we predict a sharp transition in the SMBH flaring diet beyond which all observable disruptions arise from evolved stars, accompanied by a dramatic cutoff in the overall tidal disruption flaring rate. Black holes less massive than this limiting mass scale will show observable flares from both main-sequence and evolved stars, with giants contributing up to 10% of the event rate. The relative fractions of stars disrupted at different evolutionary states can constrain the properties and distributions of stars in galactic nuclei other than our own.

THE ARDUOUS JOURNEY TO BLACK HOLE FORMATION IN POTENTIAL GAMMA-RAY BURST PROGENITORS

International Nuclear Information System (INIS)

Dessart, Luc; O'Connor, Evan; Ott, Christian D.

2012-01-01

We present a quantitative study on the properties at death of fast-rotating massive stars evolved at low-metallicity—objects that are proposed as likely progenitors of long-duration γ-ray bursts (LGRBs). We perform one-dimensional+rotation stellar-collapse simulations on the progenitor models of Woosley and Heger, and critically assess their potential for the formation of a black hole and a Keplerian disk (namely, a collapsar) or a proto-magnetar. We note that theoretical uncertainties in the treatment of magnetic fields and the approximate handling of rotation compromise the accuracy of stellar-evolution models. We find that only the fastest rotating progenitors achieve sufficient compactness for black hole formation while the bulk of models possess a core density structure typical of garden-variety core-collapse supernova (SN) progenitors evolved without rotation and at solar metallicity. Of the models that do have sufficient compactness for black hole formation, most of them also retain a large amount of angular momentum in the core, making them prone to a magneto-rotational explosion, therefore preferentially leaving behind a proto-magnetar. A large progenitor angular-momentum budget is often the sole criterion invoked in the community today to assess the suitability for producing a collapsar. This simplification ignores equally important considerations such as the core compactness, which conditions black hole formation, the core angular momentum, which may foster a magneto-rotational explosion preventing black hole formation, or the metallicity and the residual envelope mass which must be compatible with inferences from observed LGRB/SNe. Our study suggests that black hole formation is non-trivial, that there is room for accommodating both collapsars and proto-magnetars as LGRB progenitors, although proto-magnetars seem much more easily produced by current stellar-evolutionary models.

THE ARDUOUS JOURNEY TO BLACK HOLE FORMATION IN POTENTIAL GAMMA-RAY BURST PROGENITORS

Energy Technology Data Exchange (ETDEWEB)

Dessart, Luc [Laboratoire d' Astrophysique de Marseille, Universite Aix-Marseille and CNRS, UMR7326, 38 rue Frederic Joliot-Curie, 13388 Marseille (France); O' Connor, Evan; Ott, Christian D., E-mail: Luc.Dessart@oamp.fr, E-mail: evanoc@tapir.caltech.edu, E-mail: cott@tapir.caltech.edu [TAPIR, Mailcode 350-17, California Institute of Technology, Pasadena, CA 91125 (United States)

2012-07-20

We present a quantitative study on the properties at death of fast-rotating massive stars evolved at low-metallicity-objects that are proposed as likely progenitors of long-duration {gamma}-ray bursts (LGRBs). We perform one-dimensional+rotation stellar-collapse simulations on the progenitor models of Woosley and Heger, and critically assess their potential for the formation of a black hole and a Keplerian disk (namely, a collapsar) or a proto-magnetar. We note that theoretical uncertainties in the treatment of magnetic fields and the approximate handling of rotation compromise the accuracy of stellar-evolution models. We find that only the fastest rotating progenitors achieve sufficient compactness for black hole formation while the bulk of models possess a core density structure typical of garden-variety core-collapse supernova (SN) progenitors evolved without rotation and at solar metallicity. Of the models that do have sufficient compactness for black hole formation, most of them also retain a large amount of angular momentum in the core, making them prone to a magneto-rotational explosion, therefore preferentially leaving behind a proto-magnetar. A large progenitor angular-momentum budget is often the sole criterion invoked in the community today to assess the suitability for producing a collapsar. This simplification ignores equally important considerations such as the core compactness, which conditions black hole formation, the core angular momentum, which may foster a magneto-rotational explosion preventing black hole formation, or the metallicity and the residual envelope mass which must be compatible with inferences from observed LGRB/SNe. Our study suggests that black hole formation is non-trivial, that there is room for accommodating both collapsars and proto-magnetars as LGRB progenitors, although proto-magnetars seem much more easily produced by current stellar-evolutionary models.

Ultrafast Electron Dynamics in Solar Energy Conversion.

Science.gov (United States)

Ponseca, Carlito S; Chábera, Pavel; Uhlig, Jens; Persson, Petter; Sundström, Villy

2017-08-23

Electrons are the workhorses of solar energy conversion. Conversion of the energy of light to electricity in photovoltaics, or to energy-rich molecules (solar fuel) through photocatalytic processes, invariably starts with photoinduced generation of energy-rich electrons. The harvesting of these electrons in practical devices rests on a series of electron transfer processes whose dynamics and efficiencies determine the function of materials and devices. To capture the energy of a photogenerated electron-hole pair in a solar cell material, charges of opposite sign have to be separated against electrostatic attractions, prevented from recombining and being transported through the active material to electrodes where they can be extracted. In photocatalytic solar fuel production, these electron processes are coupled to chemical reactions leading to storage of the energy of light in chemical bonds. With the focus on the ultrafast time scale, we here discuss the light-induced electron processes underlying the function of several molecular and hybrid materials currently under development for solar energy applications in dye or quantum dot-sensitized solar cells, polymer-fullerene polymer solar cells, organometal halide perovskite solar cells, and finally some photocatalytic systems.

Analysis of residual transverse stresses in a thick UD glass/polyester pultruded profile using hole drilling with strain gage and digital image correlation

Science.gov (United States)

Yuksel, Onur; Baran, Ismet; Ersoy, Nuri; Akkerman, Remko

2018-05-01

Process induced stresses inherently exist in fiber reinforced polymer composites particularly in thick parts due to the presence of non-uniform cure, shrinkage and thermal expansion/contraction during manufacturing. In order to increase the reliability and the performance of the composite materials, process models are developed to predict the residual stress formation. The accuracy of the process models is dependent on the geometrical (micro to macro), material and process parameters as well as the numerical implementation. Therefore, in order to have reliable process modelling framework, there is a need for validation and if necessary calibration of the developed models. This study focuses on measurement of the transverse residual stresses in a relatively thick pultruded profile (20×20 mm) made of glass/polyester. Process-induced residual stresses in the middle of the profile are examined with different techniques which have never been applied for transverse residual stresses in thick unidirectional composites. Hole drilling method with strain gage and digital image correlation are employed. Strain values measured from measurements are used in a finite element model (FEM) to simulate the hole drilling process and predict the residual stress level. The measured released strain is found to be approximately 180 μm/m from the strain gage. The tensile residual stress at the core of the profile is estimated approximately as 7-10 MPa. Proposed methods and measured values in this study will enable validation and calibration of the process models based on the residual stresses.

Dynamics of Coulomb correlations in semiconductors in high magnetic fields

International Nuclear Information System (INIS)

Fromer, Neil Alan

2002-01-01

Current theories have been successful in explaining many nonlinear optical experiments in undoped semiconductors. However, these theories require a ground state which is assumed to be uncorrelated. Strongly correlated systems of current interest, such as a two dimensional electron gas in a high magnetic field, cannot be explained in this manner because the correlations in the ground state and the low energy collective excitations cause a breakdown of the conventional techniques. We perform ultrafast time-resolved four-wave mixing on $n$-modulation doped quantum wells, which contain a quasi-two dimensional electron gas, in a large magnetic field, when only a single Landau level is excited and also when two levels are excited together. We find evidence for memory effects and as strong coupling between the Landau levels induced by the electron gas. We compare our results with simulations based on a new microscopic approach capable of treating the collective effects and correlations of the doped electrons, and find a good qualitative agreement. By looking at the individual contributions to the model, we determine that the unusual correlation effects seen in the experiments are caused by the scattering of photo-excited electron-hole pairs with the electron gas, leading to new excited states which are not present in undoped semiconductors, and also by exciton-exciton interactions mediated by the long-lived collective excitations of the electron gas, inter-Landau level magnetoplasmons

Theoretical studies on core-level spectra of solids

International Nuclear Information System (INIS)

Kotani, Akio

1995-01-01

I present a review on theoretical studies of core-level spectra (CLS) in solids. In CLS, the dynamical response of outer electrons to a core hole is reflected through the screening of core hole potential. Impurity Anderson model (IAM) or cluster model is successfully applied to the analysis of X-ray photoemission spectra (XPS) and X-ray absorption spectra (XAS) in f and d electron systems, where the f and d electron states are hybridized with the other valence or conduction electron states. The effect of the core-hole potential in the final state of XPS and XAS plays an important role, as well as the solid state hybridization and intra-atomic multiplet coupling effects. As typical examples, the calculated results for XPS of rare-earth compounds and transition metal compounds are shown, and some discussions are given. As a subject of remarkable progress with high brightness synchrotron radiation sources, I discuss some theoretical aspects of X-ray emission spectra (XES) and their resonant enhancement at the X-ray absorption threshold. Some experimental data and their theoretical analysis are also given. (author)

Hydrostatic-pressure effects on the correlated electron-hole transition energies in GaAs-Ga{sub 1-x}Al{sub x}As semiconductor quantum wells

Energy Technology Data Exchange (ETDEWEB)

Raigoza, N. [Instituto de Fisica, Universidad de Antioquia, AA 1226, Medellin (Colombia); Instituto de Fisica, Unicamp, CP 6165, Campinas, Sao Paulo, 13083-970 (Brazil); Duque, C.A. [Instituto de Fisica, Universidad de Antioquia, AA 1226, Medellin (Colombia); Reyes-Gomez, E. [Dept. of Theor. Physics, Univ. of Havana, San Lazaro y L, Vedado 10400, Havana (Cuba); Instituto de Fisica, Unicamp, CP 6165, Campinas, Sao Paulo, 13083-970 (Brazil); Oliveira, L.E. [Instituto de Fisica, Unicamp, CP 6165, Campinas, Sao Paulo, 13083-970 (Brazil)

2006-03-01

The effects of hydrostatic pressure on the correlated e-h transition energies in single GaAs-Ga{sub 1-x}Al{sub x}As quantum wells are calculated via a variational procedure, in the framework of the effective-mass and non-degenerate parabolic-band approximations. The valence-band anisotropy is included in our theoretical model by using different hole masses in different spatial directions. Both heavy- and light-hole exciton energies are obtained, and correlated e-h transition energies are found in good agreement with available experimental measurements. (copyright 2006 WILEY-VCH Verlag GmbH and Co. KGaA, Weinheim) (orig.)

Dependence of Core and Extended Flux on Core Dominance ...

Indian Academy of Sciences (India)

Abstract. Based on two extragalactic radio source samples, the core dominance parameter is calculated, and the correlations between the core/extended flux density and core dominance parameter are investi- gated. When the core dominance parameter is lower than unity, it is linearly correlated with the core flux density, ...

Effect of strong correlations on the high energy anomaly in hole- and electron-doped high-T{sub c} superconductors

Energy Technology Data Exchange (ETDEWEB)

Moritz, B; Johnston, S; Greven, M; Shen, Z-X; Devereaux, T P [Stanford Institute for Materials and Energy Science, SLAC National Accelerator Laboratory and Stanford University, Stanford, CA 94305 (United States); Schmitt, F; Meevasana, W; Motoyama, E M [Geballe Laboratory for Advanced Materials, Stanford University, Stanford, CA 94305 (United States); Lu, D H [Stanford Synchrotron Radiation Lightsource, SLAC National Accelerator Laboratory, Menlo Park, CA 94025 (United States); Kim, C [Institute of Physics and Applied Physics, Yonsei University, Seoul 120-749 (Korea, Republic of); Scalettar, R T [Physics Department, University of California-Davis, Davis, CA 95616 (United States)], E-mail: moritzb@slac.stanford.edu

2009-09-15

Recently, angle-resolved photoemission spectroscopy (ARPES) has been used to highlight an anomalously large band renormalization at high binding energies in cuprate superconductors: the high energy 'waterfall' or high energy anomaly (HEA). This paper demonstrates, using a combination of new ARPES measurements and quantum Monte Carlo simulations, that the HEA is not simply the by-product of matrix element effects, but rather represents a cross-over from a quasi-particle band at low binding energies near the Fermi level to valence bands at higher binding energy, assumed to be of strong oxygen character, in both hole- and electron-doped cuprates. While photoemission matrix elements clearly play a role in changing the aesthetic appearance of the band dispersion, i.e. the 'waterfall'-like behavior, they provide an inadequate description for the physics that underlies the strong band renormalization giving rise to the HEA. Model calculations of the single-band Hubbard Hamiltonian showcase the role played by correlations in the formation of the HEA and uncover significant differences in the HEA energy scale for hole- and electron-doped cuprates. In addition, this approach properly captures the transfer of spectral weight accompanying both hole and electron doping in a correlated material and provides a unifying description of the HEA across both sides of the cuprate phase diagram.

First experience from in-core sensor validation based on correlation and neuro-fuzzy techniques

International Nuclear Information System (INIS)

Figedy, S.

2011-01-01

In this work new types of nuclear reactor in-core sensor validation methods are outlined. The first one is based on combination of correlation coefficients and mutual information indices, which reflect the correlation of signals in linear and nonlinear regions. The method may be supplemented by wavelet transform based signal features extraction and pattern recognition by artificial neural networks and also fuzzy logic based decision making. The second one is based on neuro-fuzzy modeling of residuals between experimental values and their theoretical counterparts obtained from the reactor core simulator calculations. The first experience with this approach is described and further improvements to enhance the outcome reliability are proposed (Author)

NuSTAR Reveals Relativistic Reflection but no Ultra-fast Outflow in the Quasar PG1211+143

DEFF Research Database (Denmark)

Zoghbi, A.; Miller, J. M.; Walton, D. J.

2015-01-01

We report on four epochs of observations of the quasar PG 1211+143 using NuSTAR. The net exposure time is 300 ks. Prior work on this source found suggestive evidence of an ultra-fast outflow ( UFO) in the Fe K band with a velocity of approximately 0.1c. The putative flow would carry away a high...... a broad Fe K emission line and Compton back-scattering curvature. The data offer only weak constraints on the spin of the black hole. A careful search for UFOs shows no significant absorption feature above 90% confidence. The limits are particularly tight when relativistic reflection is included. We...

Tilt and shift mode stability in a spheromak with a flux core

Energy Technology Data Exchange (ETDEWEB)

Finn, J.M.; Jardin, S.C.

1984-07-01

The stability of spheromak equilibria with a flux core, or reversal coil, is studied by means of an ideal MHD code. Results depend critically upon whether the flux hole region (the current free area just inside the separatrix) is treated as perfectly conducting plasma or as vacuum. This indicates that the tilt and shift modes persist as resistive instabilities if they are stable in ideal MHD. Specifically, for nonoptimally shaped equilibria, the flux core must nearly touch the current channel if the flux hole is vacuum, whereas the core may be slightly outside the separatrix if the flux hole has conducting plasma. A larger margin exists for optimally shaped equilibria.

Drilling and the associated drillhole measurements of the pilot hole ONK-PH7

International Nuclear Information System (INIS)

Oehberg, A.; Kemppainen, K.; Lampinen, H.; Niemonen, J.; Poelloenen, J.; Rouhiainen, P.; Rautio, T.; Tarvainen, A.-M.

2007-12-01

The construction of the ONKALO access tunnel started in September 2004 at Olkiluoto. Most of the investigations related to the construction of the access tunnel aim to ensure successful excavations, reinforcement and sealing. Pilot holes are drillholes, which are core drilled along the tunnel profile. The length of the pilot holes typically varies from several tens of metres to a couple of hundred metres. The pilot holes are aimed to confirm the quality of the rock mass for tunnel construction, and in particular to identify water conductive fractured zones and to provide information that could result in modifications of the existing construction plans. The pilot hole ONK-PH7 was drilled from chainage 1880 to chainage 1980.31 in February 2007. The length of the hole is 100.31 m. The aim during the drilling work was to orient core samples as much as possible. The deviation of the drillhole was measured during and after the drilling phase. Electric conductivity was measured from the collected returning water samples. Logging of the core samples included the following parameters: lithology, foliation, fracturing, fracture frequency, RQD, fractured zones, core loss and weathering. The rock mechanical logging was based on Q-classification. The tests to determine rock strength and deformation properties were made with a Rock Tester-equipment. Difference Flow method was used for the determination of hydraulic conductivity in fractures and fractured zones in the drillhole. The overlapping i.e. the detailed flow logging mode was used. Besides flow logging Single Point Resistance (SPR), Electric Conductivity (EC) and temperature of the drillhole water were also measured. The flow logging was performed with 0.5 m section length and with 0.1 m depth increment. Water loss measurements were conducted between the hole depth of 1.18 m and the hole bottom. Geophysical logging and optical imaging of the pilot hole included the fieldwork of all surveys, the integration of the data as

NNWSI [Nevada Nuclear Waste Storage Investigations] hole histories: UE-29a No. 1, UE-29a No. 2

International Nuclear Information System (INIS)

1986-11-01

This report is a compilation of data from two hydrologic exploratory core holes drilled to help identify the area geology and hydrology. The two bore holes were drilled between September, 1981 and January, 1982 under the guidance of the US Geological Survey in Area 29, Nevada Test Site. Data presented in the hole histories include all locations, daily activities, coring records, review of hole conditions, and geophysical log lists, and microfiche copies of the geophysical logs run by the Fenix and Scisson, Inc. subcontractor

Control of Dispersion in Hollow Core Photonic Crystal Fibers

DEFF Research Database (Denmark)

Roberts, John

2007-01-01

The dispersion of hollow core photonic crystal fibers can be tailored by modifying a single ring of holes in the cladding. The dispersion can be lowered and flattened, or alternatively greatly increased, in a controlled manner.......The dispersion of hollow core photonic crystal fibers can be tailored by modifying a single ring of holes in the cladding. The dispersion can be lowered and flattened, or alternatively greatly increased, in a controlled manner....

Partial coherence in the core/halo picture of Bose-Einstein n-particle correlations

OpenAIRE

Csorgo, T.; Lorstad, B.; Schmidt-Sorensen, J.; Ster, A.

1998-01-01

We study the influence of a possible coherent component in the boson source on the two-, three- and $n$-particle correlation functions in a generalized core/halo type of boson-emitting source. In particular, a simple formula is presented for the strengh of the $n$-particle correlation functions for such systems. Graph rules are obtained to evaluate the correlation functions of arbitrary high order. The importance of experimental determination of the 4-th and 5-th order Bose-Einstein correlati...

Ultrafast photoinduced structure phase transition in antimony single crystals

NARCIS (Netherlands)

Fausti, Daniele; Misochko, Oleg V.; van Loosdrecht, Paul H. M.

2009-01-01

Picosecond Raman scattering is used to study the photoinduced ultrafast dynamics in Peierls distorted antimony. We find evidence for an ultrafast nonthermal reversible structural phase transition. Most surprisingly, we find evidence that this transition evolves toward a lower symmetry in contrast to

Alteration in the IRDP drill hole compared with other drill holes in Iceland

Science.gov (United States)

Kristmannsdóttir, Hrefna

1982-08-01

The overall alteration pattern in the drill hole at Reydarfjördur is very similar to alteration patterns observed in Icelandic geothermal areas and in low-grade metamorphosed basalts in deep crustal sections elsewhere in Iceland. However more detail is obtained by the study of the IRDP drill core than by study of drill cuttings sampled in previous drill holes in Iceland. A comparatively high fossil thermal gradient is obtained at Reydarfjördur by a combination of mineral stability data and the observed occurence of secondary minerals. This high gradient is consistent with the measured dike dilation at the drill site and the location of the drill site adjacent to a central volcano.

Progress in ultrafast intense laser science

CERN Document Server

Yamanouchi, Kaoru; Mathur, Deepak

2014-01-01

The PUILS series delivers up-to-date reviews of progress in Ultrafast Intense Laser Science, a newly emerging interdisciplinary research field spanning atomic and molecular physics, molecular science, and optical science, which has been stimulated by the recent developments in ultrafast laser technologies. Each volume compiles peer-reviewed articles authored by researchers at the forefront of each their own subfields of UILS. Every chapter opens with an overview of the topics to be discussed, so that researchers unfamiliar to the subfield, as well as graduate students, can grasp the importance

Establishing a relation between the mass and the spin of stellar-mass black holes.

Science.gov (United States)

Banerjee, Indrani; Mukhopadhyay, Banibrata

2013-08-09

Stellar mass black holes (SMBHs), forming by the core collapse of very massive, rapidly rotating stars, are expected to exhibit a high density accretion disk around them developed from the spinning mantle of the collapsing star. A wide class of such disks, due to their high density and temperature, are effective emitters of neutrinos and hence called neutrino cooled disks. Tracking the physics relating the observed (neutrino) luminosity to the mass, spin of black holes (BHs) and the accretion rate (M) of such disks, here we establish a correlation between the spin and mass of SMBHs at their formation stage. Our work shows that spinning BHs are more massive than nonspinning BHs for a given M. However, slowly spinning BHs can turn out to be more massive than spinning BHs if M at their formation stage was higher compared to faster spinning BHs.

1.4 GHz on the Fundamental Plane of black hole activity

Science.gov (United States)

Saikia, Payaswini; Körding, Elmar; Dibi, Salome

2018-06-01

The Fundamental Plane (FP) of black hole activity is an empirical relationship between the O III/X-ray luminosity depicting the accretion power, the radio luminosity as a probe of the instantaneous jet power and the mass of the black hole. For the first time, we use the 1.4 GHz FIRST radio luminosities on the optical FP, to investigate whether or not Faint Images of the Radio Sky at Twenty-Centimetres (FIRST) fluxes can trace nuclear activity. We use an SDSS-FIRST cross-correlated sample of 10 149 active galaxies and analyse their positioning on the optical FP. We focus on various reasons that can cause the discrepancy between the observed FIRST radio fluxes and the theoretically expected core radio fluxes, and show that FIRST fluxes are heavily contaminated by non-nuclear, extended components and other environmental factors. We show that the subsample of `compact sources', which should have negligible lobe contribution, statistically follow the FP when corrected for relativistic beaming, while all the other sources lie above the plane. The sample of low-ionization nuclear emission-line regions (LINERs), which should have negligible lobe and beaming contribution, also follow the FP. A combined fit of the low-luminosity AGN and the X-ray binaries, with the LINERs, results in the relation log LR = 0.77 log L_{O III} + 0.69 log M. Assuming that the original FP relation is correct, we conclude that 1.4 GHz FIRST fluxes do not trace the pure `core' jet and instantaneous nuclear activity in the AGN, and one needs to be careful while using it on the FP of black hole activity.

Ultrafast THz Saturable Absorption in Doped Semiconductors

DEFF Research Database (Denmark)

Turchinovich, Dmitry; Hoffmann, Matthias C.

2011-01-01

We demonstrate ultrafast THz saturable absorption in n-doped semiconductors by nonlinear THz time-domain spectroscopy. This effect is caused by the semiconductor conductivity modulation due to electron heating and satellite-valley scattering in strong THz fields.......We demonstrate ultrafast THz saturable absorption in n-doped semiconductors by nonlinear THz time-domain spectroscopy. This effect is caused by the semiconductor conductivity modulation due to electron heating and satellite-valley scattering in strong THz fields....

Ultrafast Ultrasound Imaging With Cascaded Dual-Polarity Waves.

Science.gov (United States)

Zhang, Yang; Guo, Yuexin; Lee, Wei-Ning

2018-04-01

Ultrafast ultrasound imaging using plane or diverging waves, instead of focused beams, has advanced greatly the development of novel ultrasound imaging methods for evaluating tissue functions beyond anatomical information. However, the sonographic signal-to-noise ratio (SNR) of ultrafast imaging remains limited due to the lack of transmission focusing, and thus insufficient acoustic energy delivery. We hereby propose a new ultrafast ultrasound imaging methodology with cascaded dual-polarity waves (CDWs), which consists of a pulse train with positive and negative polarities. A new coding scheme and a corresponding linear decoding process were thereby designed to obtain the recovered signals with increased amplitude, thus increasing the SNR without sacrificing the frame rate. The newly designed CDW ultrafast ultrasound imaging technique achieved higher quality B-mode images than coherent plane-wave compounding (CPWC) and multiplane wave (MW) imaging in a calibration phantom, ex vivo pork belly, and in vivo human back muscle. CDW imaging shows a significant improvement in the SNR (10.71 dB versus CPWC and 7.62 dB versus MW), penetration depth (36.94% versus CPWC and 35.14% versus MW), and contrast ratio in deep regions (5.97 dB versus CPWC and 5.05 dB versus MW) without compromising other image quality metrics, such as spatial resolution and frame rate. The enhanced image qualities and ultrafast frame rates offered by CDW imaging beget great potential for various novel imaging applications.

Drilling and associated drillhole measurements of the pilot hole ONK-PH10

International Nuclear Information System (INIS)

Mancini, P.; Karttunen, P.; Lokkila, M.; Pekkanen, J.; Poellaenen, J.; Tarvainen, A.-M.; Toropainen, V.; Kosunen, P.; Pere, T.

2010-08-01

The construction of the ONKALO access tunnel started in September 2004 at Olkiluoto. Most of the investigations related to the construction of the access tunnel aim to ensure successful excavations, reinforcement and sealing. Pilot holes are drillholes, which are core drilled along the tunnel profile. The length of the pilot holes typically varies from several tens of metres to a couple of hundred metres. The pilot holes are aimed to confirm the quality of the rock mass for tunnel construction, and in particular to identify water conductive fractured zones and to provide information that could result in modifications of the existing construction plans. The pilot hole ONK-PH10 was drilled from chainage 3459 to chainage 3639 in March 2009. The length of the hole is 180.00 metres. The drilling was done as orientated core drilling. The deviation of the drillhole was measured during and after the drilling phase. Electric conductivity was measured from the collected returning water samples. Logging of the core samples included the following parameters: lithology, foliation, fracturing, fracture frequency, RQD, fractured zones, core loss, and weathering. The rock mechanical logging was based on Q-classification. The test to determine rock strength and deformation were made with Rock Tester -equipment. Water conductivity of the fractures or fractured zones was measured by Posiva Flow Log equipment. The measurements were done in two phases. During flow measurements also grounding resistance electric conductivity and temperature were measured. In flow logging test, sections of 0.5 m with increments of 0.1 m were used. Water loss measurements were conducted in the hole section 3.70-180.00 m dhd. Geophysical logging and optical imaging of the pilot hole included the fieldwork of all surveys, the integration of the data as well as interpretation of the acoustic and drillhole radar data. One of the objectives of the geochemical study was to get information of the composition of

Jet outflow and gamma-ray emission correlations in S5 0716+714

International Nuclear Information System (INIS)

Rani, B.; Krichbaum, T. P.; Marscher, A. P.

2014-01-01

Here, using millimeter very long baseline interferometry (VLBI) observations of the BL Lac object S5 0716+714 from August 2008 to September 2013, we investigate variations in the core flux density and orientation of the sub-parsec scale jet, i.e. position angle. The γ-ray data obtained by the Fermi Large Area Telescope are used to investigate the high-energy flux variations over the same time period. For the first time in any blazar, we report a significant correlation between the γ-ray flux variations and the position angle variations in the VLBI jet. The cross-correlation analysis also indicates a positive correlation such that the mm-VLBI core flux density variations are delayed with respect to the γ-ray flux by 82±32 days. This suggests that the high-energy emission is coming from a region located ≥(3.8±1.9) parsecs upstream of the mm-VLBI core (closer to the central black hole). Lastly, these results imply that the observed inner jet morphology has a strong connection with the observed γ-ray flares.

Highly efficient fluorescence sensing with hollow core photonic crystal fibers

DEFF Research Database (Denmark)

Smolka, Stephan; Barth, Michael; Benson, Oliver

2008-01-01

We investigate hollow core photonic crystal fibers for ultra-sensitive fluorescence detection by selectively infiltrating the central hole with fluorophores. Dye concentrations down to 10(-9) M can be detected using only nanoliter sample volumes.......We investigate hollow core photonic crystal fibers for ultra-sensitive fluorescence detection by selectively infiltrating the central hole with fluorophores. Dye concentrations down to 10(-9) M can be detected using only nanoliter sample volumes....

Generation of ultrafast pulse via combined effects of stimulated

Indian Academy of Sciences (India)

A project of ultrafast pulse generation has been presented and demonstrated by utilizing the combined nonlinear effects of stimulated Raman scattering (SRS) and non-degenerate two-photon absorption (TPA) based on silicon nanophotonic chip, in which a continuous wave (CW) and an ultrafast dark pulse are ...

The use of geological data from pilot holes for predicting FPI (full perimeter intersection) fractures

International Nuclear Information System (INIS)

Joutsen, A.

2012-02-01

Posiva Oy is responsible for preparation of final disposal of spent nuclear fuel in Olkiluoto. The knowledge about existing network of fractures is important for the safety and feasibility of the final repository. The bedrock properties essential for safety case are analyzed in investigations of Rock Suitability Criteria (RSC). One subtask in RSC is avoidance of large (long) fractures adjacent to disposal holes. The long fractures have been defined in tunnel mapping to indicate tunnel cross-cutting fractures (TCF) or full perimeter intersections (FPI). The purpose for this study was to evaluate the possibility of recognizing FPIs from drill cores by their geological properties. The study was carried out by correlating FPIs mapped from the ONKALO tunnel to the pilot holes logging data with a view of finding out which fracture in the pilot hole corresponds to the FPI in the tunnel. It was also estimated what kind of geological properties does FPIs commonly have in the tunnel and how does these properties differ from the FPI correlated pilot hole fractures. The data sources for this study are the pilot holes from ONK-PH8 to ONK-PH14 and the systematic geological mapping data. The FPIs used in this study usually follow the general trends of the fracturing in the Olkiluoto bedrock. The fracture surface profiles are principally undulating and a striation can be often seen on the fracture surfaces. The FPIs are frequently moderately to intensely altered with diverse filling mineralogy and thick fracture fillings in comparison to the regular fractures. The FPI correlated pilot hole fractures have slightly different properties in comparison to the FPIs. These fractures have wider range of different fracture surface profiles and are slightly less altered than the FPIs. Filling mineralogy follows the trends of the FPIs but filling thicknesses are thinner. These differences probably occur because of the variable uncertainties related to the correlation and to the fact that the

The use of geological data from pilot holes for predicting FPI (full perimeter intersection) fractures

Energy Technology Data Exchange (ETDEWEB)

Joutsen, A.

2012-02-15

Posiva Oy is responsible for preparation of final disposal of spent nuclear fuel in Olkiluoto. The knowledge about existing network of fractures is important for the safety and feasibility of the final repository. The bedrock properties essential for safety case are analyzed in investigations of Rock Suitability Criteria (RSC). One subtask in RSC is avoidance of large (long) fractures adjacent to disposal holes. The long fractures have been defined in tunnel mapping to indicate tunnel cross-cutting fractures (TCF) or full perimeter intersections (FPI). The purpose for this study was to evaluate the possibility of recognizing FPIs from drill cores by their geological properties. The study was carried out by correlating FPIs mapped from the ONKALO tunnel to the pilot holes logging data with a view of finding out which fracture in the pilot hole corresponds to the FPI in the tunnel. It was also estimated what kind of geological properties does FPIs commonly have in the tunnel and how does these properties differ from the FPI correlated pilot hole fractures. The data sources for this study are the pilot holes from ONK-PH8 to ONK-PH14 and the systematic geological mapping data. The FPIs used in this study usually follow the general trends of the fracturing in the Olkiluoto bedrock. The fracture surface profiles are principally undulating and a striation can be often seen on the fracture surfaces. The FPIs are frequently moderately to intensely altered with diverse filling mineralogy and thick fracture fillings in comparison to the regular fractures. The FPI correlated pilot hole fractures have slightly different properties in comparison to the FPIs. These fractures have wider range of different fracture surface profiles and are slightly less altered than the FPIs. Filling mineralogy follows the trends of the FPIs but filling thicknesses are thinner. These differences probably occur because of the variable uncertainties related to the correlation and to the fact that the

Ultrafast Outflows: Galaxy-scale Active Galactic Nucleus Feedback

Science.gov (United States)

Wagner, A. Y.; Umemura, M.; Bicknell, G. V.

2013-01-01

We show, using global three-dimensional grid-based hydrodynamical simulations, that ultrafast outflows (UFOs) from active galactic nuclei (AGNs) result in considerable feedback of energy and momentum into the interstellar medium (ISM) of the host galaxy. The AGN wind interacts strongly with the inhomogeneous, two-phase ISM consisting of dense clouds embedded in a tenuous, hot, hydrostatic medium. The outflow floods through the intercloud channels, sweeps up the hot ISM, and ablates and disperses the dense clouds. The momentum of the UFO is primarily transferred to the dense clouds via the ram pressure in the channel flow, and the wind-blown bubble evolves in the energy-driven regime. Any dependence on UFO opening angle disappears after the first interaction with obstructing clouds. On kpc scales, therefore, feedback by UFOs operates similarly to feedback by relativistic AGN jets. Negative feedback is significantly stronger if clouds are distributed spherically rather than in a disk. In the latter case, the turbulent backflow of the wind drives mass inflow toward the central black hole. Considering the common occurrence of UFOs in AGNs, they are likely to be important in the cosmological feedback cycles of galaxy formation.

ULTRAFAST OUTFLOWS: GALAXY-SCALE ACTIVE GALACTIC NUCLEUS FEEDBACK

Energy Technology Data Exchange (ETDEWEB)

Wagner, A. Y.; Umemura, M. [Center for Computational Sciences, University of Tsukuba, 1-1-1 Tennodai, Tsukuba, Ibaraki, 305-8577 (Japan); Bicknell, G. V., E-mail: ayw@ccs.tsukuba.ac.jp [Research School of Astronomy and Astrophysics, Australian National University, ACT 2611 (Australia)

2013-01-20

We show, using global three-dimensional grid-based hydrodynamical simulations, that ultrafast outflows (UFOs) from active galactic nuclei (AGNs) result in considerable feedback of energy and momentum into the interstellar medium (ISM) of the host galaxy. The AGN wind interacts strongly with the inhomogeneous, two-phase ISM consisting of dense clouds embedded in a tenuous, hot, hydrostatic medium. The outflow floods through the intercloud channels, sweeps up the hot ISM, and ablates and disperses the dense clouds. The momentum of the UFO is primarily transferred to the dense clouds via the ram pressure in the channel flow, and the wind-blown bubble evolves in the energy-driven regime. Any dependence on UFO opening angle disappears after the first interaction with obstructing clouds. On kpc scales, therefore, feedback by UFOs operates similarly to feedback by relativistic AGN jets. Negative feedback is significantly stronger if clouds are distributed spherically rather than in a disk. In the latter case, the turbulent backflow of the wind drives mass inflow toward the central black hole. Considering the common occurrence of UFOs in AGNs, they are likely to be important in the cosmological feedback cycles of galaxy formation.

ULTRAFAST OUTFLOWS: GALAXY-SCALE ACTIVE GALACTIC NUCLEUS FEEDBACK

International Nuclear Information System (INIS)

Wagner, A. Y.; Umemura, M.; Bicknell, G. V.

2013-01-01

We show, using global three-dimensional grid-based hydrodynamical simulations, that ultrafast outflows (UFOs) from active galactic nuclei (AGNs) result in considerable feedback of energy and momentum into the interstellar medium (ISM) of the host galaxy. The AGN wind interacts strongly with the inhomogeneous, two-phase ISM consisting of dense clouds embedded in a tenuous, hot, hydrostatic medium. The outflow floods through the intercloud channels, sweeps up the hot ISM, and ablates and disperses the dense clouds. The momentum of the UFO is primarily transferred to the dense clouds via the ram pressure in the channel flow, and the wind-blown bubble evolves in the energy-driven regime. Any dependence on UFO opening angle disappears after the first interaction with obstructing clouds. On kpc scales, therefore, feedback by UFOs operates similarly to feedback by relativistic AGN jets. Negative feedback is significantly stronger if clouds are distributed spherically rather than in a disk. In the latter case, the turbulent backflow of the wind drives mass inflow toward the central black hole. Considering the common occurrence of UFOs in AGNs, they are likely to be important in the cosmological feedback cycles of galaxy formation.

Dynamics-based selective 2D 1H/1H chemical shift correlation spectroscopy under ultrafast MAS conditions

Science.gov (United States)

Zhang, Rongchun; Ramamoorthy, Ayyalusamy

2015-05-01

Dynamics plays important roles in determining the physical, chemical, and functional properties of a variety of chemical and biological materials. However, a material (such as a polymer) generally has mobile and rigid regions in order to have high strength and toughness at the same time. Therefore, it is difficult to measure the role of mobile phase without being affected by the rigid components. Herein, we propose a highly sensitive solid-state NMR approach that utilizes a dipolar-coupling based filter (composed of 12 equally spaced 90° RF pulses) to selectively measure the correlation of 1H chemical shifts from the mobile regions of a material. It is interesting to find that the rotor-synchronized dipolar filter strength decreases with increasing inter-pulse delay between the 90° pulses, whereas the dipolar filter strength increases with increasing inter-pulse delay under static conditions. In this study, we also demonstrate the unique advantages of proton-detection under ultrafast magic-angle-spinning conditions to enhance the spectral resolution and sensitivity for studies on small molecules as well as multi-phase polymers. Our results further demonstrate the use of finite-pulse radio-frequency driven recoupling pulse sequence to efficiently recouple weak proton-proton dipolar couplings in the dynamic regions of a molecule and to facilitate the fast acquisition of 1H/1H correlation spectrum compared to the traditional 2D NOESY (Nuclear Overhauser effect spectroscopy) experiment. We believe that the proposed approach is beneficial to study mobile components in multi-phase systems, such as block copolymers, polymer blends, nanocomposites, heterogeneous amyloid mixture of oligomers and fibers, and other materials.

Dynamics-based selective 2D 1H/1H chemical shift correlation spectroscopy under ultrafast MAS conditions

International Nuclear Information System (INIS)

Zhang, Rongchun; Ramamoorthy, Ayyalusamy

2015-01-01

Dynamics plays important roles in determining the physical, chemical, and functional properties of a variety of chemical and biological materials. However, a material (such as a polymer) generally has mobile and rigid regions in order to have high strength and toughness at the same time. Therefore, it is difficult to measure the role of mobile phase without being affected by the rigid components. Herein, we propose a highly sensitive solid-state NMR approach that utilizes a dipolar-coupling based filter (composed of 12 equally spaced 90° RF pulses) to selectively measure the correlation of 1 H chemical shifts from the mobile regions of a material. It is interesting to find that the rotor-synchronized dipolar filter strength decreases with increasing inter-pulse delay between the 90° pulses, whereas the dipolar filter strength increases with increasing inter-pulse delay under static conditions. In this study, we also demonstrate the unique advantages of proton-detection under ultrafast magic-angle-spinning conditions to enhance the spectral resolution and sensitivity for studies on small molecules as well as multi-phase polymers. Our results further demonstrate the use of finite-pulse radio-frequency driven recoupling pulse sequence to efficiently recouple weak proton-proton dipolar couplings in the dynamic regions of a molecule and to facilitate the fast acquisition of 1 H/ 1 H correlation spectrum compared to the traditional 2D NOESY (Nuclear Overhauser effect spectroscopy) experiment. We believe that the proposed approach is beneficial to study mobile components in multi-phase systems, such as block copolymers, polymer blends, nanocomposites, heterogeneous amyloid mixture of oligomers and fibers, and other materials

Linear and ultrafast nonlinear plasmonics of single nano-objects

Science.gov (United States)

Crut, Aurélien; Maioli, Paolo; Vallée, Fabrice; Del Fatti, Natalia

2017-03-01

Single-particle optical investigations have greatly improved our understanding of the fundamental properties of nano-objects, avoiding the spurious inhomogeneous effects that affect ensemble experiments. Correlation with high-resolution imaging techniques providing morphological information (e.g. electron microscopy) allows a quantitative interpretation of the optical measurements by means of analytical models and numerical simulations. In this topical review, we first briefly recall the principles underlying some of the most commonly used single-particle optical techniques: near-field, dark-field, spatial modulation and photothermal microscopies/spectroscopies. We then focus on the quantitative investigation of the surface plasmon resonance (SPR) of metallic nano-objects using linear and ultrafast optical techniques. While measured SPR positions and spectral areas are found in good agreement with predictions based on Maxwell’s equations, SPR widths are strongly influenced by quantum confinement (or, from a classical standpoint, surface-induced electron scattering) and, for small nano-objects, cannot be reproduced using the dielectric functions of bulk materials. Linear measurements on single nano-objects (silver nanospheres and gold nanorods) allow a quantification of the size and geometry dependences of these effects in confined metals. Addressing the ultrafast response of an individual nano-object is also a powerful tool to elucidate the physical mechanisms at the origin of their optical nonlinearities, and their electronic, vibrational and thermal relaxation processes. Experimental investigations of the dynamical response of gold nanorods are shown to be quantitatively modeled in terms of modifications of the metal dielectric function enhanced by plasmonic effects. Ultrafast spectroscopy can also be exploited to unveil hidden physical properties of more complex nanosystems. In this context, two-color femtosecond pump-probe experiments performed on individual

Observation of Internal Photoinduced Electron and Hole Separation in Hybrid Two-Dimentional Perovskite Films.

Science.gov (United States)

Liu, Junxue; Leng, Jing; Wu, Kaifeng; Zhang, Jun; Jin, Shengye

2017-02-01

Two-dimensional (2D) organolead halide perovskites are promising for various optoelectronic applications. Here we report a unique spontaneous charge (electron/hole) separation property in multilayered (BA) 2 (MA) n-1 Pb n I 3n+1 (BA = CH 3 (CH 2 ) 3 NH 3 + , MA = CH 3 NH 3 + ) 2D perovskite films by studying the charge carrier dynamics using ultrafast transient absorption and photoluminescence spectroscopy. Surprisingly, the 2D perovskite films, although nominally prepared as "n = 4", are found to be mixture of multiple perovskite phases, with n = 2, 3, 4 and ≈ ∞, that naturally align in the order of n along the direction perpendicular to the substrate. Driven by the band alignment between 2D perovskites phases, we observe consecutive photoinduced electron transfer from small-n to large-n phases and hole transfer in the opposite direction on hundreds of picoseconds inside the 2D film of ∼358 nm thickness. This internal charge transfer efficiently separates electrons and holes to the upper and bottom surfaces of the films, which is a unique property beneficial for applications in photovoltaics and other optoelectronics devices.

Drilling and the associated drillhole measurements of the pilot hole ONK-PH5

International Nuclear Information System (INIS)

Oehberg, A.; Hirvonen, H.; Jurvanen, T.; Kemppainen, K.; Mustonen, A.; Niemonen, J.; Poellaenen, J.; Rouhiainen, P.; Rautio, T.

2006-09-01

The construction of the ONKALO access tunnel started in September 2004 at Olkiluoto. Most of the investigations related to the construction of the access tunnel aim to ensure successful excavations, reinforcement and sealing. Pilot holes are drillholes, which are core drilled along the tunnel profile. The length of the pilot holes typically varies from several tens of metres to a couple of hundred metres. The pilot holes are aimed to confirm the quality of the rock mass for tunnel construction, and in particular to identify water conductive fractured zones and to provide information that could result in modifications of the existing construction plans. The pilot hole ONK-PH5 was drilled from chainage 991.4 to chainage 1194 in January 2006. The length of the hole is 202.64 m and the vertical depth of the hole from zero level is about 88.2-107.5 m. The aim during the drilling work was to orient core samples as much as possible. The deviation of the drillhole was measured during and after the drilling phase. One steering operation by wedging was made at the hole depth of 128.58 metres. Electric conductivity was measured from the collected returning water samples. Logging of the core samples included the following parameters: lithology, foliation, fracturing, fracture frequency, RQD, fractured zones, core loss and weathering. The rock mechanical logging was based on Q-classification. The tests to determine rock strength and deformation properties were made with a Rock Tester-equipment. Due to high inflow (c. 200 L/min) mainly from the depth section 56-58 metres no geophysical surveys were carried out in the hole. Flow logging was carried out only from 58 metres to the bottom of the hole. Difference Flow method was used for the determination of hydraulic conductivity in fractures and fractured zones in the drillhole. The overlapping i.e. the detailed flow logging mode was used. The flow logging was performed with 0.5 m section length and with 0.1 m depth increment. Flow

Density functional theory calculations of energy-loss carbon near-edge spectra of small diameter armchair and zigzag nanotubes: Core-hole, curvature, and momentum-transfer orientation effects

International Nuclear Information System (INIS)

Titantah, J.T.; Lamoen, D.; Jorissen, K.

2004-01-01

We perform density functional theory calculations on a series of armchair and zigzag nanotubes of diameters less than 1 nm using the all-electron full-potential(-linearized)-augmented-plane-wave method. Emphasis is laid on the effects of curvature, the electron-beam orientation, and the inclusion of the core hole on the carbon electron-energy-loss K edge. The electron-energy-loss near-edge spectra of all the studied tubes show strong curvature effects compared to that of flat graphene. The curvature-induced π-σ hybridization is shown to have a more drastic effect on the electronic properties of zigzag tubes than on those of armchair tubes. We show that the core-hole effect must be accounted for in order to correctly reproduce electron-energy-loss measurements. We also find that the energy-loss near-edge spectra of these carbon systems are dominantly dipole selected and that they can be expressed simply as a proportionality with the local momentum projected density of states, thus portraying the weak energy dependence of the transition matrix elements. Compared to graphite, we report a reduction in the anisotropy as seen on the energy-loss near-edge spectra of carbon nanotubes

Interface engineered ferrite@ferroelectric core-shell nanostructures: A facile approach to impart superior magneto-electric coupling

Science.gov (United States)

Abraham, Ann Rose; Raneesh, B.; Das, Dipankar; Oluwafemi, Oluwatobi Samuel; Thomas, Sabu; Kalarikkal, Nandakumar

2018-04-01

The electric field control of magnetism in multiferroics is attractive for the realization of ultra-fast and miniaturized low power device applications like nonvolatile memories. Room temperature hybrid multiferroic heterostructures with core-shell (0-0) architecture (ferrite core and ferroelectric shell) were developed via a two-step method. High-Resolution Transmission Electron Microscopy (HRTEM) images confirm the core-shell structure. The temperature dependant magnetization measurements and Mossbauer spectra reveal superparamagnetic nature of the core-shell sample. The ferroelectric hysteresis loops reveal leaky nature of the samples. The results indicate the promising applications of the samples for magneto-electric memories and spintronics.

Unification of X-ray Winds in Seyfert Galaxies: From Ultra-fast Outflows to Warm Absorbers

Science.gov (United States)

Tombesi, F.; Cappi, M.; Reeves, J. N.; Nemmen, R. S.; Braito, V.; Gaspari, M.; Reynolds, C. S.

2013-01-01

The existence of ionized X-ray absorbing layers of gas along the line of sight to the nuclei of Seyfert galaxies is a well established observational fact. This material is systematically outflowing and shows a large range in parameters. However, its actual nature and dynamics are still not clear. In order to gain insights into these important issues we performed a literature search for papers reporting the parameters of the soft X-ray warm absorbers (WAs) in 35 type 1 Seyferts and compared their properties to those of the ultra-fast outflows (UFOs) detected in the same sample. The fraction of sources with WAs is >60 per cent, consistent with previous studies. The fraction of sources with UFOs is >34 per cent, >67 per cent of which also show WAs. The large dynamic range obtained when considering all the absorbers together, spanning several orders of magnitude in ionization, column, velocity and distance allows us, for the first time, to investigate general relations among them. In particular, we find significant correlations indicating that the closer the absorber is to the central black hole, the higher the ionization, column, outflow velocity and consequently the mechanical power. In all the cases, the absorbers continuously populate the whole parameter space, with the WAs and the UFOs lying always at the two ends of the distribution. These evidence strongly suggest that these absorbers, often considered of different types, could actually represent parts of a single large-scale stratified outflow observed at different locations from the black hole. The UFOs are likely launched from the inner accretion disc and the WAs at larger distances, such as the outer disc and/or torus. We argue that the observed parameters and correlations are, to date, consistent with both radiation pressure through Compton scattering and magnetohydrodynamic processes contributing to the outflow acceleration, the latter playing a major role. Most of the absorbers, especially the UFOs, show

Detection of coronary artery calcification by ultrafast CT and correlation with angiography

International Nuclear Information System (INIS)

Zhang Shaoxiong; Dai Ruping; Lu Bin

1997-01-01

To investigate the relationship between coronary calcification and significant coronary stenosis ninety patients including 81 men and 9 women were studied asithage ranging from 27∼72 years (mean, 58 years). All patients had both ultrafast CT (UFCT) examination and coronary angiography within one month. Single slice mode with ECG gating and thickness of 3 mm were used in UFCT scan. Selected coronary angiography was performed by the Judkins technique. Among 160 vessels in which coronary calcifications were identified, 74% had significant coronary stenosis (>50% stenosis), and 77% of 154 vessels with significant coronary stenosis had calcification demonstrable by UFCT. In the younger age group the sensitivity of calcification for evaluating stenosis of coronary artery was lower and the specificity was generally higher than those in the elderly group. UFCT is a promising procedure for detecting coronary arterial disease, since this examination has high sensitivity and specificity, easy to conduct, noninvasive, and widely applicable for screening a large population

Gamma ray bursts of black hole universe

Science.gov (United States)

Zhang, T. X.

2015-07-01

Slightly modifying the standard big bang theory, Zhang recently developed a new cosmological model called black hole universe, which has only a single postulate but is consistent with Mach's principle, governed by Einstein's general theory of relativity, and able to explain existing observations of the universe. In the previous studies, we have explained the origin, structure, evolution, expansion, cosmic microwave background radiation, quasar, and acceleration of black hole universe, which grew from a star-like black hole with several solar masses through a supermassive black hole with billions of solar masses to the present state with hundred billion-trillions of solar masses by accreting ambient matter and merging with other black holes. This study investigates gamma ray bursts of black hole universe and provides an alternative explanation for the energy and spectrum measurements of gamma ray bursts according to the black hole universe model. The results indicate that gamma ray bursts can be understood as emissions of dynamic star-like black holes. A black hole, when it accretes its star or merges with another black hole, becomes dynamic. A dynamic black hole has a broken event horizon and thus cannot hold the inside hot (or high-frequency) blackbody radiation, which flows or leaks out and produces a GRB. A star when it collapses into its core black hole produces a long GRB and releases the gravitational potential energy of the star as gamma rays. A black hole that merges with another black hole produces a short GRB and releases a part of their blackbody radiation as gamma rays. The amount of energy obtained from the emissions of dynamic star-like black holes are consistent with the measurements of energy from GRBs. The GRB energy spectra derived from this new emission mechanism are also consistent with the measurements.

Feed-forward motor control of ultrafast, ballistic movements.

Science.gov (United States)

Kagaya, K; Patek, S N

2016-02-01

To circumvent the limits of muscle, ultrafast movements achieve high power through the use of springs and latches. The time scale of these movements is too short for control through typical neuromuscular mechanisms, thus ultrafast movements are either invariant or controlled prior to movement. We tested whether mantis shrimp (Stomatopoda: Neogonodactylus bredini) vary their ultrafast smashing strikes and, if so, how this control is achieved prior to movement. We collected high-speed images of strike mechanics and electromyograms of the extensor and flexor muscles that control spring compression and latch release. During spring compression, lateral extensor and flexor units were co-activated. The strike initiated several milliseconds after the flexor units ceased, suggesting that flexor activity prevents spring release and determines the timing of strike initiation. We used linear mixed models and Akaike's information criterion to serially evaluate multiple hypotheses for control mechanisms. We found that variation in spring compression and strike angular velocity were statistically explained by spike activity of the extensor muscle. The results show that mantis shrimp can generate kinematically variable strikes and that their kinematics can be changed through adjustments to motor activity prior to the movement, thus supporting an upstream, central-nervous-system-based control of ultrafast movement. Based on these and other findings, we present a shishiodoshi model that illustrates alternative models of control in biological ballistic systems. The discovery of feed-forward control in mantis shrimp sets the stage for the assessment of targets, strategic variation in kinematics and the role of learning in ultrafast animals. © 2016. Published by The Company of Biologists Ltd.

Effect of correlation in the 3d/sup n/ core on the resonance transition in Cu II

International Nuclear Information System (INIS)

Fischer, C.F.; Glass, R.

1979-01-01

A preliminary report is presented on the effect of correlation in the 3d/sup n/ core on the 3d 10 1 S → 3d 9 4p 1 P f value by use of the multiconfiguration (MC) Hartree-Fock procedure. A common orbital basis was used for correlation in the core, with virtual orbitals determined variationally for the initial state. Three different approximations were used: a single-configuration approximation for both initial and final state, a MC approximation for 3d 10 correlation in the initial state and a single configuration for the final state, and MC approximations for both initial and final states. Some preliminary f values for the 3d 10 1 S → 3d 9 4p 1 P transition are tabulated. Comparison of calculated with experimental values indicates that correlation in the 3d 9 core of the final state is needed to obtain the correct transition energy to bring the length and velocity forms into good agreement with themselves and experiment, and that the multiplet strength for the transition is not greatly affected by correlation. 1 table

Microscopic origin of black hole reentrant phase transitions

Science.gov (United States)

Zangeneh, M. Kord; Dehyadegari, A.; Sheykhi, A.; Mann, R. B.

2018-04-01

Understanding the microscopic behavior of the black hole ingredients has been one of the important challenges in black hole physics during the past decades. In order to shed some light on the microscopic structure of black holes, in this paper, we explore a recently observed phenomenon for black holes namely reentrant phase transition, by employing the Ruppeiner geometry. Interestingly enough, we observe two properties for the phase behavior of small black holes that leads to reentrant phase transition. They are correlated and they are of the interaction type. For the range of pressure in which the system underlies reentrant phase transition, it transits from the large black holes phase to the small one which possesses higher correlation than the other ranges of pressures. On the other hand, the type of interaction between small black holes near the large/small transition line differs for usual and reentrant phase transitions. Indeed, for the usual case, the dominant interaction is repulsive whereas for the reentrant case we encounter an attractive interaction. We show that in the reentrant phase transition case, the small black holes behave like a bosonic gas whereas in the usual phase transition case, they behave like a quantum anyon gas.

Simultaneous effects of electron-hole correlation, hydrostatic pressure, and temperature on the third harmonic generation in parabolic GaAs quantum dots

International Nuclear Information System (INIS)

Duque, C. M.; Mora-Ramos, M. E.; Duque, C. A.

2011-01-01

The combined effects of electron-hole correlation, hydrostatic pressure, and temperature on the third harmonic generation in disk-shaped parabolic GaAs quantum dots are studied under the density matrix formalism and the effective mass approximation. Two well-defined regimes are discussed: (1) the strong-confinement regime, where the Coulomb interaction between the electron and hole is neglected and (2) the weak-confinement regime where the parabolic confinement term is neglected and the system reaches the limit of a hydrogenic problem. The results show that the third harmonic-generation coefficient is strongly dependent on the localization of the electron-hole pair. Also, that by using external perturbations like hydrostatic pressure or by considering the temperature effects it is possible to induce a blue-shift and/or red-shift on the resonant peaks of the third harmonic generation coefficient.

THE M BH-L SPHEROID RELATION AT HIGH AND LOW MASSES, THE QUADRATIC GROWTH OF BLACK HOLES, AND INTERMEDIATE-MASS BLACK HOLE CANDIDATES

International Nuclear Information System (INIS)

Graham, Alister W.; Scott, Nicholas

2013-01-01

From a sample of 72 galaxies with reliable supermassive black hole masses M bh , we derive the M bh -(host spheroid luminosity, L) relation for (1) the subsample of 24 core-Sérsic galaxies with partially depleted cores, and (2) the remaining subsample of 48 Sérsic galaxies. Using K s -band Two Micron All Sky Survey data, we find the near-linear relation M bh ∝L 1.10±0.20 K s for the core-Sérsic spheroids thought to be built in additive dry merger events, while we find the relation M bh ∝L 2.73±0.55 K s for the Sérsic spheroids built from gas-rich processes. After converting literature B-band disk galaxy magnitudes into inclination- and dust-corrected bulge magnitudes, via a useful new equation presented herein, we obtain a similar result. Unlike with the M bh -(velocity dispersion) diagram, which is also updated here using the same galaxy sample, it remains unknown whether barred and non-barred Sérsic galaxies are offset from each other in the M bh -L diagram. While black hole feedback has typically been invoked to explain what was previously thought to be a nearly constant M bh /M Spheroid mass ratio of ∼0.2%, we advocate that the near-linear M bh -L and M bh -M Spheroid relations observed at high masses may have instead arisen largely from the additive dry merging of galaxies. We argue that feedback results in a dramatically different scaling relation, such that black hole mass scales roughly quadratically with the spheroid mass in Sérsic galaxies. We therefore introduce a revised cold-gas 'quasar' mode feeding equation for semi-analytical models to reflect what we dub the quadratic growth of black holes in Sérsic galaxies built amidst gas-rich processes. Finally, we use our new Sérsic M bh -L equations to predict the masses of candidate intermediate mass black holes in almost 50 low-luminosity spheroids containing active galactic nuclei, finding many masses between that of stellar mass black holes and supermassive black holes.

Ultrafast Nonlinear Signal Processing in Silicon Waveguides

DEFF Research Database (Denmark)

Oxenløwe, Leif Katsuo; Mulvad, Hans Christian Hansen; Hu, Hao

2012-01-01

We describe recent demonstrations of exploiting highly nonlinear silicon waveguides for ultrafast optical signal processing. We describe wavelength conversion and serial-to-parallel conversion of 640 Gbit/s data signals and 1.28 Tbit/s demultiplexing and all-optical sampling.......We describe recent demonstrations of exploiting highly nonlinear silicon waveguides for ultrafast optical signal processing. We describe wavelength conversion and serial-to-parallel conversion of 640 Gbit/s data signals and 1.28 Tbit/s demultiplexing and all-optical sampling....

Optimization and practical implementation of ultrafast 2D NMR experiments

Energy Technology Data Exchange (ETDEWEB)

Queiroz Junior, Luiz H. K., E-mail: professorkeng@gmail.com [Universidade Federal de Sao Carlos (UFSC), SP (Brazil). Departamento de Quimica; Universidade Federal de Goias (UFGO), Goiania, GO (Brazil). Inst. de Quimica; Ferreira, Antonio G. [Universidade Federal de Sao Carlos (UFSC), SP (Brazil). Departamento de Quimica; Giraudeau, Patrick [Universite de Nantes (France). CNRS, Chimie et Interdisciplinarite: Synthese, Analyse, Modelisation

2013-09-01

Ultrafast 2D NMR is a powerful methodology that allows recording of a 2D NMR spectrum in a fraction of second. However, due to the numerous non-conventional parameters involved in this methodology its implementation is no trivial task. Here, an optimized experimental protocol is carefully described to ensure efficient implementation of ultrafast NMR. The ultrafast spectra resulting from this implementation are presented based on the example of two widely used 2D NMR experiments, COSY and HSQC, obtained in 0.2 s and 41 s, respectively. (author)

All-optical temporal integration of ultrafast pulse waveforms.

Science.gov (United States)

Park, Yongwoo; Ahn, Tae-Jung; Dai, Yitang; Yao, Jianping; Azaña, José

2008-10-27

An ultrafast all-optical temporal integrator is experimentally demonstrated. The demonstrated integrator is based on a very simple and practical solution only requiring the use of a widely available all-fiber passive component, namely a reflection uniform fiber Bragg grating (FBG). This design allows overcoming the severe speed (bandwidth) limitations of the previously demonstrated photonic integrator designs. We demonstrate temporal integration of a variety of ultrafast optical waveforms, including Gaussian, odd-symmetry Hermite Gaussian, and (odd-)symmetry double pulses, with temporal features as fast as ~6-ps, which is about one order of magnitude faster than in previous photonic integration demonstrations. The developed device is potentially interesting for a multitude of applications in all-optical computing and information processing, ultrahigh-speed optical communications, ultrafast pulse (de-)coding, shaping and metrology.

Heat flow at the proposed Appalachian Ultradeep Core Hole (ADCOH) Site: Tectonic implications

Science.gov (United States)

Costain, John K.; Decker, Edward R.

The heat flow in northwestern South Carolina at the Appalachian Ultradeep Core Hole (ADCOH) site area is approximately 55 mW/m². This data supplements other data to the east in the Piedmont and Atlantic Coastal Plain provinces where heat flows > 55 mW/m² are characteristic of post- and late-synmetamorphic granitoids. Piedmont heat flow and heat generation data for granites, metagranites, and one Slate Belt site, in a zone approximately parallel to major structural Appalachian trends, define a linear relation. Tectonic truncation of heat-producing crust at a depth of about 8 km (a depth equal to the slope of the heat flow-heat production line) is proposed to explain the linear relation. Using the value of reduced heat flow estimated from this empirical relation, and assuming thicknesses of heat-producing crust defined by new ADCOH seismic data, the heat flow and heat production at the ADCOH site are consistent with a depth to the base of the Inner Piedmont crystalline allochthon of about 5.5 km. Seismic data at the ADCOH site confirm that the Inner Piedmont is tectonically truncated at about 5.5 km by the Blue Ridge master decollement. Temperatures at 10 km at the ADCOH site are predicted to be less than 200 °C.

Probing charge transfer dynamics in self-assembled monolayers by core hole clock approach

International Nuclear Information System (INIS)

Zharnikov, Michael

2015-01-01

This article reviews recent progress in the application of core hole clock approach in the framework of resonant Auger electron spectroscopy to the monomolecular assembles of alkyl, oligophenyl, and oligo(phenylene–ethynylene) based molecules on Au(1 1 1) substrates, referring mostly to the work by the author et al. The major goal was to study electron transfer (ET) dynamics in these systems serving as prototypes of molecular electronics (ME) devices. The ET pathway to the conductive substrate was unambiguously defined by resonant excitation of the nitrile tailgroup attached to the molecular backbone. Characteristic ET times within the femtosecond domain were determined, along with the attenuation factors for the ET dynamics, analogous to the case of the static transport. The above parameters were found to exhibit strong dependence on the character of the molecular orbital which mediates the ET process. In addition, certain spectral features, which can be associated with an inverse ET from the molecular backbone to the excitation site, were observed upon exchange of the nitrile group by strongly electronegative nitro moiety. The reported results represent a valuable input for theory and a certain potential for applications such as ME devices where optimization of ET can have significant technological impact.

Drilling and the associated drillhole measurements of the pilot hole ONK-PH4

International Nuclear Information System (INIS)

Oehberg, A.; Heikkinen, E.; Hirvonen, H.; Kemppainen, K.; Majapuro, J.; Niemonen, J.; Poellaenen, J.; Rouhiainen, P.; Rautio, T.

2006-09-01

The construction of the ONKALO access tunnel started in September 2004 at Olkiluoto. Most of the investigations related to the construction of the access tunnel aim to ensure successful excavations, reinforcement and sealing. Pilot holes are drillholes, which are core drilled along the tunnel profile. The length of the pilot holes typically varies from several tens of metres to a couple of hundred metres. The pilot holes are mostly aimed to confirm the quality of the rock mass for tunnel construction, and in particular to identify water conductive fractured zones and to provide information that could result in modifications of the existing construction plans. The pilot hole ONK-PH4 was drilled in October 2005. The length of the hole is 96.01 metres. During the drilling work core samples were oriented as much as possible. The deviation of the hole was measured during and after the drilling phase. Electric conductivity was measured from the collected returning water samples. Geological logging of the core samples included the following parameters: lithology, foliation, fracturing, fracture frequency, RQD, fractured zones, core loss and weathering. The rock mechanical logging was based on Q-classification. The tests to determine rock strength and deformation properties were made with a Rock Tester-equipment. Difference Flow method was used for the determination of hydraulic conductivity in fractures and fractured zones in the hole. The overlapping i.e. the detailed flow logging mode was used. The flow logging was performed with 0.5 m section length and with 0.1 m depth increment. Water loss tests (Lugeon tests) were used to give background information for the grouting design. Geophysical logging and optical imaging of the pilot hole PH4 included the field work of all surveys, the integration of the data as well as interpretation of the acoustic and drillhole radar data. One of the objectives of the geochemical study was to get information of composition of ONKALO

Triplet exciton dissociation and electron extraction in graphene-templated pentacene observed with ultrafast spectroscopy.

Science.gov (United States)

McDonough, Thomas J; Zhang, Lushuai; Roy, Susmit Singha; Kearns, Nicholas M; Arnold, Michael S; Zanni, Martin T; Andrew, Trisha L

2017-02-08

We compare the ultrafast dynamics of singlet fission and charge generation in pentacene films grown on glass and graphene. Pentacene grown on graphene is interesting because it forms large crystals with the long axis of the molecules "lying-down" (parallel to the surface). At low excitation fluence, spectra for pentacene on graphene contain triplet absorptions at 507 and 545 nm and no bleaching at 630 nm, which we show is due to the orientation of the pentacene molecules. We perform the first transient absorption anisotropy measurements on pentacene, observing negative anisotropy of the 507 and 545 nm peaks, consistent with triplet absorption. A broad feature at 853 nm, observed on both glass and graphene, is isotropic, suggesting hole absorption. At high fluence, there are additional features, whose kinetics and anisotropies are not explained by heating, that we assign to charge generation; we propose a polaron pair absorption at 614 nm. The lifetimes are shorter at high fluence for both pentacene on glass and graphene, indicative of triplet-triplet annihilation that likely enhances charge generation. The anisotropy decays more slowly for pentacene on graphene than on glass, in keeping with the smaller domain size observed via atomic force microscopy. Coherent acoustic phonons are observed for pentacene on graphene, which is a consequence of more homogeneous domains. Measuring the ultrafast dynamics of pentacene as a function of molecular orientation, fluence, and polarization provides new insight to previous spectral assignments.

Short-Range Correlated Magnetic Core-Shell CrO2/Cr2O3 Nanorods: Experimental Observations and Theoretical Considerations

Directory of Open Access Journals (Sweden)

Ashish C. Gandhi

2018-05-01

Full Text Available With the evolution of synthesis and the critical characterization of core-shell nanostructures, short-range magnetic correlation is of prime interest in employing their properties to develop novel devices and widespread applications. In this regard, a novel approach of the magnetic core-shell saturated magnetization (CSSM cylinder model solely based on the contribution of saturated magnetization in one-dimensional CrO2/Cr2O3 core-shell nanorods (NRs has been developed and applied for the determination of core-diameter and shell-thickness. The nanosized effect leads to a short-range magnetic correlation of ferromagnetic core-CrO2 extracted from CSSM, which can be explained using finite size scaling method. The outcome of this study is important in terms of utilizing magnetic properties for the critical characterization of core-shell nanomagnetic materials.

The dynamical fingerprint of core scouring in massive elliptical galaxies

International Nuclear Information System (INIS)

Thomas, J.; Saglia, R. P.; Bender, R.; Erwin, P.; Fabricius, M.

2014-01-01

The most massive elliptical galaxies have low-density centers or cores that differ dramatically from the high-density centers of less massive ellipticals and bulges of disk galaxies. These cores have been interpreted as the result of mergers of supermassive black hole binaries, which depopulate galaxy centers by gravitationally slingshotting central stars toward large radii. Such binaries naturally form in mergers of luminous galaxies. Here, we analyze the population of central stellar orbits in 11 massive elliptical galaxies that we observed with the integral field spectrograph SINFONI at the European Southern Observatory Very Large Telescope. Our dynamical analysis is orbit-based and includes the effects of a central black hole, the mass distribution of the stars, and a dark matter halo. We show that the use of integral field kinematics and the inclusion of dark matter is important to conclude on the distribution of stellar orbits in galaxy centers. Six of our galaxies are core galaxies. In these six galaxies, but not in the galaxies without cores, we detect a coherent lack of stars on radial orbits in the core region and a uniform excess of radial orbits outside of it: when scaled by the core radius r b , the radial profiles of the classical anisotropy parameter β(r) are nearly identical in core galaxies. Moreover, they quantitatively match the predictions of black hole binary simulations, providing the first convincing dynamical evidence for core scouring in the most massive elliptical galaxies.

Ultrafast electron diffraction studies of optically excited thin bismuth films

International Nuclear Information System (INIS)

Rajkovic, Ivan

2008-01-01

This thesis contains work on the design and the realization of an experimental setup capable of providing sub-picosecond electron pulses for ultrafast electron diffraction experiments, and performing the study of ultrafast dynamics in bismuth after optical excitation using this setup. (orig.)

Ultrafast electron diffraction studies of optically excited thin bismuth films

Energy Technology Data Exchange (ETDEWEB)

Rajkovic, Ivan

2008-10-21

This thesis contains work on the design and the realization of an experimental setup capable of providing sub-picosecond electron pulses for ultrafast electron diffraction experiments, and performing the study of ultrafast dynamics in bismuth after optical excitation using this setup. (orig.)

Black hole solution in the framework of arctan-electrodynamics

Science.gov (United States)

Kruglov, S. I.

An arctan-electrodynamics coupled with the gravitational field is investigated. We obtain the regular black hole solution that at r →∞ gives corrections to the Reissner-Nordström solution. The corrections to Coulomb’s law at r →∞ are found. We evaluate the mass of the black hole that is a function of the dimensional parameter β introduced in the model. The magnetically charged black hole was investigated and we have obtained the magnetic mass of the black hole and the metric function at r →∞. The regular black hole solution is obtained at r → 0 with the de Sitter core. We show that there is no singularity of the Ricci scalar for electrically and magnetically charged black holes. Restrictions on the electric and magnetic fields are found that follow from the requirement of the absence of superluminal sound speed and the requirement of a classical stability.

Two quasi-particle excitations with particle-hole core polarization in even-even single closed shell nuclei

International Nuclear Information System (INIS)

Gillet, V.; Giraud, B.; Rho, M.

1976-01-01

The energy levels and transition properties of the even-even N=28, 50 isotones and Z=28, 50, 82 isotopes are calculated in the framework of the Tamm-Dancoff and Random Phase Approximation, with an effective central interaction in an extended space consisting of two quasi-particle configurations for the open shell and particle-hole configurations for the closed core. Using the results of the Inverse Gap Equation Method, practically all the necessary input data (single quasi-particle energies, force strength) are extracted from the odd-mass nuclei. The ratios of the force components are kept at fixed values for all studied nuclei and no effective charge is used. An overall excellent agreement is obtained for the energies of the vibrational states. On the other hand, while the transition properties of the 3 - states are always well reproduced, those of the 2 + and 4 + states are often too small by about one order of magnitude [fr

Drilling and associated drillhole measurements of the pilot hole ONK-PH9

International Nuclear Information System (INIS)

Karttunen, P.; Pekkanen, J.; Poellaenen, J.; Tarvainen, A.-M.; Toropainen, V.; Lamminmaeki, T.; Kosunen, P.

2010-01-01

The construction of the ONKALO access tunnel started in September 2004 at Olkiluoto. Most of the investigations related to the construction of the access tunnel aim to ensure successful excavations, reinforcement and sealing. Pilot holes are drillholes, which are core drilled along the tunnel profile. The length of the pilot holes typically varies from several tens of metres to a couple of hundred metres. The pilot holes are aimed to confirm the quality of the rock mass for tunnel construction, and in particular to identify water conductive fractured zones and to provide information that could result in modifications of the existing construction plans. The pilot hole ONK-PH9 was drilled from chainage 3263 to chainage 3413.27 in November 2008. The length of the hole is 150.3 metres. The aim during the drilling work was to orient core samples as much as possible. The deviation of the drillhole was measured during and after the drilling phase. Electric conductivity was measured from the collected returning water samples. Hydraulic conductivity of the fractures or fractured zones was measured by Posiva Flow Log equipment. The measurements were done in two phases. During flow measurements also electric conductivity, grounding resistance and temperature were measured. In flow logging test sections of 0.5 m and increments of 0.1 m were used. The water loss measurements were performed after drilling was completed by the drilling company. Logging of the core samples included the following parameters: lithology, foliation, fracturing, fracture frequency, RQD, fractured zones, core loss, and weathering. The rock mechanical logging was based on Q-classification. The rock strength and deformation were determined with Rock Tester equipment. Geophysical logging and optical imaging of the pilot hole included the fieldwork of all surveys, the integration of the data as well as interpretation of the acoustic and drillhole radar data. One of the objectives of the geochemical study

Entropy of black holes with multiple horizons

Science.gov (United States)

He, Yun; Ma, Meng-Sen; Zhao, Ren

2018-05-01

We examine the entropy of black holes in de Sitter space and black holes surrounded by quintessence. These black holes have multiple horizons, including at least the black hole event horizon and a horizon outside it (cosmological horizon for de Sitter black holes and "quintessence horizon" for the black holes surrounded by quintessence). Based on the consideration that the two horizons are not independent each other, we conjecture that the total entropy of these black holes should not be simply the sum of entropies of the two horizons, but should have an extra term coming from the correlations between the two horizons. Different from our previous works, in this paper we consider the cosmological constant as the variable and employ an effective method to derive the explicit form of the entropy. We also try to discuss the thermodynamic stabilities of these black holes according to the entropy and the effective temperature.

Impact of correlations between core configurations for the evaluation of nuclear data uncertainty propagation for reactivity

International Nuclear Information System (INIS)

Frosio, T.; Bonaccorsi, T.; Blaise, P.

2017-01-01

The precise estimation of Pearson correlations, also called 'representativity' coefficients, between core configurations is a fundamental quantity for properly assessing the nuclear data (ND) uncertainties propagation on integral parameters such as k-eff, power distributions, or reactivity coefficients. In this paper, a traditional adjoint method is used to propagate ND uncertainty on reactivity and reactivity coefficients and estimate correlations between different states of the core. We show that neglecting those correlations induces a loss of information in the final uncertainty. We also show that using approximate values of Pearson does not lead to an important error of the model. This calculation is made for reactivity at the beginning of life and can be extended to other parameters during depletion calculations. (authors)

The Yucca Mountain Project prototype air-coring test, U12g tunnel, Nevada test site

International Nuclear Information System (INIS)

Ray, J.M.; Newsom, J.C.

1994-12-01

The Prototype Air-Coring Test was conducted at the Nevada Test Site (NTS) G-Tunnel facility to evaluate standard coring techniques, modified slightly for air circulation, for use in testing at a prospective nuclear waste repository at Yucca Mountain, Nevada. Air-coring technology allows sampling of subsurface lithology with minimal perturbation to ambient characteristic such as that required for exploratory holes near aquifers, environmental applications, and site characterization work. Two horizontal holes were cored, one 50 ft long and the other 150 ft long, in densely welded fractured tuff to simulate the difficult drilling conditions anticipated at Yucca Mountain. Drilling data from seven holes on three other prototype tests in nonwelded tuff were also collected for comparison. The test was used to establish preliminary standards of performance for drilling and dust collection equipment and to assess procedural efficiencies. The Longyear-38 drill achieved 97% recovery for HQ-size core (-2.5 in.), and the Atlas Copco dust collector (DCT-90) captured 1500 lb of fugitive dust in a mine environment with only minor modifications. Average hole production rates were 6-8 ft per 6-h shift in welded tuff and almost 20 ft per shift on deeper holes in nonwelded tuff. Lexan liners were successfully used to encapsulate core samples during the coring process and protect core properties effectively. The Prototype Air-Coring Test demonstrated that horizontal air coring in fractured welded tuff (to at least 150 ft) can be safely accomplished by proper selection, integration, and minor modification of standard drilling equipment, using appropriate procedures and engineering controls. The test also indicated that rig logistics, equipment, and methods need improvement before attempting a large-scale dry drilling program at Yucca Mountain

A PSF-Shape-Based Beamforming Strategy for Robust 2D Motion Estimation in Ultrafast Data

Directory of Open Access Journals (Sweden)

Anne E. C. M. Saris

2018-03-01

Full Text Available This paper presents a framework for motion estimation in ultrafast ultrasound data. It describes a novel approach for determining the sampling grid for ultrafast data based on the system’s point-spread-function (PSF. As a consequence, the cross-correlation functions (CCF used in the speckle tracking (ST algorithm will have circular-shaped peaks, which can be interpolated using a 2D interpolation method to estimate subsample displacements. Carotid artery wall motion and parabolic blood flow simulations together with rotating disk experiments using a Verasonics Vantage 256 are used for performance evaluation. Zero-degree plane wave data were acquired using an ATL L5-12 (fc = 9 MHz transducer for a range of pulse repetition frequencies (PRFs, resulting in 0–600 µm inter-frame displacements. The proposed methodology was compared to data beamformed on a conventionally spaced grid, combined with the commonly used 1D parabolic interpolation. The PSF-shape-based beamforming grid combined with 2D cubic interpolation showed the most accurate and stable performance with respect to the full range of inter-frame displacements, both for the assessment of blood flow and vessel wall dynamics. The proposed methodology can be used as a protocolled way to beamform ultrafast data and obtain accurate estimates of tissue motion.

Progress in ultrafast intense laser science XI

CERN Document Server

Yamanouchi, Kaoru; Martin, Philippe

2014-01-01

The PUILS series delivers up-to-date reviews of progress in Ultrafast Intense Laser Science, a newly emerging interdisciplinary research field spanning atomic and molecular physics, molecular science and optical science, which has been stimulated by the recent developments in ultrafast laser technologies. Each volume compiles peer-reviewed articles authored by researchers at the forefront of each their own subfields of UILS. Every chapter opens with an overview of the topics to be discussed, so that researchers unfamiliar to the subfield, as well as graduate students, can grasp the importance

Progress in Ultrafast Intense Laser Science II

CERN Document Server

Yamanouchi, Kaoru; Agostini, Pierre; Ferrante, Gaetano

2007-01-01

This book series addresses a newly emerging interdisciplinary research field, Ultrafast Intense Laser Science, spanning atomic and molecular physics, molecular science, and optical science. Its progress is being stimulated by the recent development of ultrafast laser technologies. Highlights of this second volume include Coulomb explosion and fragmentation of molecules, control of chemical dynamics, high-order harmonic generation, propagation and filamentation, and laser-plasma interaction. All chapters are authored by foremost experts in their fields and the texts are written at a level accessible to newcomers and graduate students, each chapter beginning with an introductory overview.

Mega-electron-volt ultrafast electron diffraction at SLAC National Accelerator Laboratory

Energy Technology Data Exchange (ETDEWEB)

Weathersby, S. P.; Brown, G.; Chase, T. F.; Coffee, R.; Corbett, J.; Eichner, J. P.; Frisch, J. C.; Fry, A. R.; Gühr, M.; Hartmann, N.; Hast, C.; Hettel, R.; Jobe, R. K.; Jongewaard, E. N.; Lewandowski, J. R.; Li, R. K., E-mail: lrk@slac.stanford.edu; Lindenberg, A. M.; Makasyuk, I.; May, J. E.; McCormick, D. [SLAC National Accelerator Laboratory, 2575 Sand Hill Road, Menlo Park, California 94025 (United States); and others

2015-07-15

Ultrafast electron probes are powerful tools, complementary to x-ray free-electron lasers, used to study structural dynamics in material, chemical, and biological sciences. High brightness, relativistic electron beams with femtosecond pulse duration can resolve details of the dynamic processes on atomic time and length scales. SLAC National Accelerator Laboratory recently launched the Ultrafast Electron Diffraction (UED) and microscopy Initiative aiming at developing the next generation ultrafast electron scattering instruments. As the first stage of the Initiative, a mega-electron-volt (MeV) UED system has been constructed and commissioned to serve ultrafast science experiments and instrumentation development. The system operates at 120-Hz repetition rate with outstanding performance. In this paper, we report on the SLAC MeV UED system and its performance, including the reciprocal space resolution, temporal resolution, and machine stability.

Cosmological production of noncommutative black holes

International Nuclear Information System (INIS)

Mann, Robert B.; Nicolini, Piero

2011-01-01

We investigate the pair creation of noncommutative black holes in a background with a positive cosmological constant. As a first step we derive the noncommutative geometry inspired Schwarzschild-de Sitter solution. By varying the mass and the cosmological constant parameters, we find several spacetimes compatible with the new solution: positive-mass spacetimes admit one cosmological horizon and two, one, or no black hole horizons, while negative-mass spacetimes have just a cosmological horizon. These new black holes share the properties of the corresponding asymptotically flat solutions, including the nonsingular core and thermodynamic stability in the final phase of the evaporation. As a second step we determine the action which generates the matter sector of gravitational field equations and we construct instantons describing the pair production of black holes and the other admissible topologies. As a result we find that for current values of the cosmological constant the de Sitter background is quantum mechanically stable according to experience. However, positive-mass noncommutative black holes and solitons would have plentifully been produced during inflationary times for Planckian values of the cosmological constant. As a special result we find that, in these early epochs of the Universe, Planck size black holes production would have been largely disfavored. We also find a potential instability for production of negative-mass solitons.

Entropy of black holes with multiple horizons

Directory of Open Access Journals (Sweden)

Yun He

2018-05-01

Full Text Available We examine the entropy of black holes in de Sitter space and black holes surrounded by quintessence. These black holes have multiple horizons, including at least the black hole event horizon and a horizon outside it (cosmological horizon for de Sitter black holes and “quintessence horizon” for the black holes surrounded by quintessence. Based on the consideration that the two horizons are not independent each other, we conjecture that the total entropy of these black holes should not be simply the sum of entropies of the two horizons, but should have an extra term coming from the correlations between the two horizons. Different from our previous works, in this paper we consider the cosmological constant as the variable and employ an effective method to derive the explicit form of the entropy. We also try to discuss the thermodynamic stabilities of these black holes according to the entropy and the effective temperature.

Connecting traces of galaxy evolution: the missing core mass-morphological fine structure relation

Science.gov (United States)

Bonfini, P.; Bitsakis, T.; Zezas, A.; Duc, P.-A.; Iodice, E.; González-Martín, O.; Bruzual, G.; González Sanoja, A. J.

2018-01-01

Deep exposure imaging of early-type galaxies (ETGs) are revealing the second-order complexity of these objects, which have been long considered uniform, dispersion-supported spheroidals. `Fine structure' features (e.g. ripples, plumes, tidal tails, rings) as well as depleted stellar cores (i.e. central light deficits) characterize a number of massive ETG galaxies, and can be interpreted as the result of galaxy-galaxy interactions. We discuss how the time-scale for the evolution of cores and fine structures are comparable, and hence it is expected that they develop in parallel after the major interaction event which shaped the ETG. Using archival data, we compare the `depleted stellar mass' (i.e. the mass missing from the depleted stellar core) against the prominence of the fine structure features, and observe that they correlate inversely. This result confirms our expectation that, while the supermassive black hole (SMBH) binary (constituted by the SMBHs of the merger progenitors) excavates the core via three-body interactions, the gravitational potential of the newborn galaxy relaxes, and the fine structures fade below detection levels. We expect the inverse correlation to hold at least within the first Gyr from the merger which created the SMBH binary; after then, the fine structure evolves independently.

Thermal barrier and support for nuclear reactor fuel core

International Nuclear Information System (INIS)

Betts, W.S. Jr.; Pickering, J.L.; Black, W.E.

1987-01-01

A nuclear reactor is described having a thermal barrier for supporting a fuel column of a nuclear reactor core within a reactor vessel having a fixed rigid metal liner. The fuel column has a refractory post extending downward. The thermal barrier comprises, in combination, a metallic core support having an interior chamber secured to the metal liner; fibrous thermal insulation material covering the metal liner and surrounding the metallic core support; means associated with the metallic core support and resting on the top for locating and supporting the full column post; and a column of ceramic material located within the interior chamber of the metallic core support, the height of the column is less than the height of the metallic core support so that the ceramic column will engage the means for locating and supporting the fuel column post only upon plastic deformation of the metallic core support; the core support comprises a metallic cylinder and the ceramic column comprises coaxially aligned ceramic pads. Each pad has a hole located within the metallic cylinder by means of a ceramic post passing through the holes in the pads

Drilling and associated Drillhole measurements of the Pilot Hole ONK-PH14

International Nuclear Information System (INIS)

Aalto, P.; Toropainen, V.; Tarvainen, A.-M.; Pekkanen, J.; Poellaenen, J.; Lamminmaeki, T.

2011-09-01

The construction of ONKALO access tunnel started in September 2004 at Olkiluoto. During the construction, investigations serving both research and construction purposes need to be done. Investigations can be done for example in so called pilot holes. Pilot holes are cored drillholes to be drilled to the tunnel profile. The length of the holes varies from some tens of metres to some hundreds of metres. The purpose of the holes is to confirm the quality of the rock mass for tunnel construction, especially to identify water conductive fractures/fractured zones and to provide information that could result in modifications of the existing construction plans. The pilot hole ONK-PH14 was drilled in June 2010. Drilling was started in chainage 4313.6. The length of the hole was 150.80 metres. The deviation of the drillhole was measured during and after the drilling. Additionally, oriented core samples were collected from the drill core and the electric conductivity of returning water was measured. Logging of the core samples included following parameters: lithology, foliation, fracturing, fracture frequency, RQD, fractured zones, core loss and weathering. The rock mechanical logging was based on Q-classification. The strength and deformation properties of the rock were defined by using Rock-Tester equipment. Hydraulic measurements were made by using the PFL DIFF (Posiva Flow log, Difference Flow Method). PFL DIFF measurements were performed with a 0.5 m section length and with 0.1 m length increments. With PFL DIFF tool the locations of transmissive fractures were detected. Simultaneously, the electric conductivity (EC) of the drillhole water and fracture specific water, temperature of the drillhole water, single point resistance (SPR) of the drillhole wall and the prevailing water pressure were measured. Water loss measurements were done after the drilling by the tool developed by Posiva. The tool was in test use during the measurements. The groundwater sample was

Drilling and associated Drillhole measurements of the Pilot Hole ONK-PH14

Energy Technology Data Exchange (ETDEWEB)

Aalto, P. (ed.); Lahti, M.; Kosunen, P.; Pere, T. [Posiva Oy, Helsinki (Finland); Toropainen, V.; Tarvainen, A.-M. [Suomen Malmi Oy, Espoo (Finland); Pekkanen, J.; Poellaenen, J. [Poeyry Finland Oy, Espoo (Finland); Lamminmaeki, T. [Teollisuuden Voima Oyj, Helsinki (Finland)

2011-08-15

The construction of ONKALO access tunnel started in September 2004 at Olkiluoto. During the construction, investigations serving both research and construction purposes need to be done. Investigations can be done for example in so called pilot holes. Pilot holes are cored drillholes to be drilled to the tunnel profile. The length of the holes varies from some tens of metres to some hundreds of metres. The purpose of the holes is to confirm the quality of the rock mass for tunnel construction, especially to identify water conductive fractures/fractured zones and to provide information that could result in modifications of the existing construction plans. The pilot hole ONK-PH14 was drilled in June 2010. Drilling was started in chainage 4313.6. The length of the hole was 150.80 metres. The deviation of the drillhole was measured during and after the drilling. Additionally, oriented core samples were collected from the drill core and the electric conductivity of returning water was measured. Logging of the core samples included following parameters: lithology, foliation, fracturing, fracture frequency, RQD, fractured zones, core loss and weathering. The rock mechanical logging was based on Q-classification. The strength and deformation properties of the rock were defined by using Rock-Tester equipment. Hydraulic measurements were made by using the PFL DIFF (Posiva Flow log, Difference Flow Method). PFL DIFF measurements were performed with a 0.5 m section length and with 0.1 m length increments. With PFL DIFF tool the locations of transmissive fractures were detected. Simultaneously, the electric conductivity (EC) of the drillhole water and fracture specific water, temperature of the drillhole water, single point resistance (SPR) of the drillhole wall and the prevailing water pressure were measured. Water loss measurements were done after the drilling by the tool developed by Posiva. The tool was in test use during the measurements. The groundwater sample was

State-Space Geometry, Statistical Fluctuations, and Black Holes in String Theory

Directory of Open Access Journals (Sweden)

Stefano Bellucci

2014-01-01

Full Text Available We study the state-space geometry of various extremal and nonextremal black holes in string theory. From the notion of the intrinsic geometry, we offer a state-space perspective to the black hole vacuum fluctuations. For a given black hole entropy, we explicate the intrinsic geometric meaning of the statistical fluctuations, local and global stability conditions, and long range statistical correlations. We provide a set of physical motivations pertaining to the extremal and nonextremal black holes, namely, the meaning of the chemical geometry and physics of correlation. We illustrate the state-space configurations for general charge extremal black holes. In sequel, we extend our analysis for various possible charge and anticharge nonextremal black holes. From the perspective of statistical fluctuation theory, we offer general remarks, future directions, and open issues towards the intrinsic geometric understanding of the vacuum fluctuations and black holes in string theory.

Geology of the UE17e drill hole, Area 17, Nevada Test Site

International Nuclear Information System (INIS)

Hodson, J.N.; Hoover, D.L.

1979-03-01

The UE17e drill hole, located at the northwest corner of Syncline Ridge, was cored from 3.05 m (10 ft) to a total depth of 914.4 m (3,000 ft) in unit J (Mississippian) of the Eleana (Devonian and Mississippian) to obtain samples for mineral, chemical, and physical-property analyses. UE17e penetrated 73.5 m (241 ft) of the quartzite subunit and 840.9 m (2,759 ft) of the argillite subunit of unit J. Less than 0.4 percent quartzite is present in the argillite subunit. Dips range from 12 0 to 18 0 . Twenty-three faults were observed in the core or on geophysical logs. Most of these faults affect only a few meters of the core and probably have displacements of a few meters. The majority of fractures are parallel to bedding planes. Fracture frequency ranges from 3.4 to 9.4 fractures per meter in the upper part of the cored interval and 1.4 to 5.9 fractures per meter in the lower part of the cored interval. The core index indicates that the lower part of the hole is more competent than the upper part. Lower competency in the upper part of the hole may be caused by weathering and/or near-surface stress relief. Physical, mechanical, and thermal property measurements indicate that bedding and fracturing are the major factors in variation of properties between samples. 17 figures, 10 tables

Carrier dynamics in graphene. Ultrafast many-particle phenomena

Energy Technology Data Exchange (ETDEWEB)

Malic, E.; Brem, S.; Jago, R. [Department of Physics, Chalmers University of Technology, Goeteborg (Sweden); Winzer, T.; Wendler, F.; Knorr, A. [Institut fuer Theoretische Physik, Technische Universitaet Berlin (Germany); Mittendorff, M.; Koenig-Otto, J.C.; Schneider, H.; Helm, M.; Winnerl, S. [Helmholtz-Zentrum Dresden-Rossendorf, Dresden (Germany); Ploetzing, T.; Neumaier, D. [Advanced Microelectronic Center Aachen, AMO GmbH, Aachen (Germany)

2017-11-15

Graphene is an ideal material to study fundamental Coulomb- and phonon-induced carrier scattering processes. Its remarkable gapless and linear band structure opens up new carrier relaxation channels. In particular, Auger scattering bridging the valence and the conduction band changes the number of charge carriers and gives rise to a significant carrier multiplication - an ultrafast many-particle phenomenon that is promising for the design of highly efficient photodetectors. Furthermore, the vanishing density of states at the Dirac point combined with ultrafast phonon-induced intraband scattering results in an accumulation of carriers and a population inversion suggesting the design of graphene-based terahertz lasers. Here, we review our work on the ultrafast carrier dynamics in graphene and Landau-quantized graphene is presented providing a microscopic view on the appearance of carrier multiplication and population inversion. (copyright 2017 by WILEY-VCH Verlag GmbH and Co. KGaA, Weinheim)

Black hole complementarity: The inside view

Directory of Open Access Journals (Sweden)

David A. Lowe

2014-10-01

Full Text Available Within the framework of black hole complementarity, a proposal is made for an approximate interior effective field theory description. For generic correlators of local operators on generic black hole states, it agrees with the exact exterior description in a region of overlapping validity, up to corrections that are too small to be measured by typical infalling observers.

WE-B-210-02: The Advent of Ultrafast Imaging in Biomedical Ultrasound

International Nuclear Information System (INIS)

Tanter, M.

2015-01-01

In the last fifteen years, the introduction of plane or diverging wave transmissions rather than line by line scanning focused beams has broken the conventional barriers of ultrasound imaging. By using such large field of view transmissions, the frame rate reaches the theoretical limit of physics dictated by the ultrasound speed and an ultrasonic map can be provided typically in tens of micro-seconds (several thousands of frames per second). Interestingly, this leap in frame rate is not only a technological breakthrough but it permits the advent of completely new ultrasound imaging modes, including shear wave elastography, electromechanical wave imaging, ultrafast doppler, ultrafast contrast imaging, and even functional ultrasound imaging of brain activity (fUltrasound) introducing Ultrasound as an emerging full-fledged neuroimaging modality. At ultrafast frame rates, it becomes possible to track in real time the transient vibrations – known as shear waves – propagating through organs. Such “human body seismology” provides quantitative maps of local tissue stiffness whose added value for diagnosis has been recently demonstrated in many fields of radiology (breast, prostate and liver cancer, cardiovascular imaging, …). Today, Supersonic Imagine company is commercializing the first clinical ultrafast ultrasound scanner, Aixplorer with real time Shear Wave Elastography. This is the first example of an ultrafast Ultrasound approach surpassing the research phase and now widely spread in the clinical medical ultrasound community with an installed base of more than 1000 Aixplorer systems in 54 countries worldwide. For blood flow imaging, ultrafast Doppler permits high-precision characterization of complex vascular and cardiac flows. It also gives ultrasound the ability to detect very subtle blood flow in very small vessels. In the brain, such ultrasensitive Doppler paves the way for fUltrasound (functional ultrasound imaging) of brain activity with unprecedented

WE-B-210-02: The Advent of Ultrafast Imaging in Biomedical Ultrasound

Energy Technology Data Exchange (ETDEWEB)

Tanter, M. [Laboratoire Ondes et Acoustique (France)

2015-06-15

In the last fifteen years, the introduction of plane or diverging wave transmissions rather than line by line scanning focused beams has broken the conventional barriers of ultrasound imaging. By using such large field of view transmissions, the frame rate reaches the theoretical limit of physics dictated by the ultrasound speed and an ultrasonic map can be provided typically in tens of micro-seconds (several thousands of frames per second). Interestingly, this leap in frame rate is not only a technological breakthrough but it permits the advent of completely new ultrasound imaging modes, including shear wave elastography, electromechanical wave imaging, ultrafast doppler, ultrafast contrast imaging, and even functional ultrasound imaging of brain activity (fUltrasound) introducing Ultrasound as an emerging full-fledged neuroimaging modality. At ultrafast frame rates, it becomes possible to track in real time the transient vibrations – known as shear waves – propagating through organs. Such “human body seismology” provides quantitative maps of local tissue stiffness whose added value for diagnosis has been recently demonstrated in many fields of radiology (breast, prostate and liver cancer, cardiovascular imaging, …). Today, Supersonic Imagine company is commercializing the first clinical ultrafast ultrasound scanner, Aixplorer with real time Shear Wave Elastography. This is the first example of an ultrafast Ultrasound approach surpassing the research phase and now widely spread in the clinical medical ultrasound community with an installed base of more than 1000 Aixplorer systems in 54 countries worldwide. For blood flow imaging, ultrafast Doppler permits high-precision characterization of complex vascular and cardiac flows. It also gives ultrasound the ability to detect very subtle blood flow in very small vessels. In the brain, such ultrasensitive Doppler paves the way for fUltrasound (functional ultrasound imaging) of brain activity with unprecedented

Quantitative ultra-fast MRI of HPMC swelling and dissolution.

Science.gov (United States)

Chen, Ya Ying; Hughes, L P; Gladden, L F; Mantle, M D

2010-08-01

For the first time quantitative Rapid Acquisition with Relaxation Enhancement (RARE) based ultra-fast two-dimensional magnetic resonance imaging has been used to follow the dissolution of hydroxypropylmethyl cellulose (HPMC) in water. Quantitative maps of absolute water concentration, spin-spin relaxation times and water self-diffusion coefficient are obtained at a spatial resolution of 469 microm in less than 3 min each. These maps allow the dynamic development of the medium release rate HPMC/water system to be followed. It is demonstrated that the evolution of the gel layer and, in particular, the gradient in water concentration across it, is significantly different when comparing the quantitative RARE sequence with a standard (nonquantitative) implementation of RARE. The total gel thickness in the axial direction grows faster than that in the radial direction and that the dry core initially expands anisotropically. Additionally, while HPMC absorbs a large amount of water during the dissolution process, the concentration gradient of water within the gel layer is relatively small. For the first time MRI evidence is presented for a transition swollen glassy layer which resides between the outer edge of the dry tablet core and the inner edge of the gel layer. (c) 2010 Wiley-Liss, Inc. and the American Pharmacists Association

In-core flow rate distribution measurement test of the JOYO irradiation core

International Nuclear Information System (INIS)

Suzuki, Toshihiro; Isozaki, Kazunori; Suzuki, Soju

1996-01-01

A flow rate distribution measurement test was carried out for the JOYO irradiation core (the MK-II core) after the 29th duty cycle operation. The main object of the test is to confirm the proper flow rate distribution at the final phase of the MK-II core. The each flow rate at the outlet of subassemblies was measured by the permanent magnetic flowmeter inserted avail of fuel exchange hole in the rotating plug. This is third test in the MK-II core, after 10 years absence from the final test (1985). Total of 550 subassemblies were exchanged and accumulated reactor operation time reached up to 38,000 hours from the previous test. As a conclusion, it confirmed that the flow rate distribution has been kept suitable in the final phase of the MK-II core. (author)

Coherent combination of ultrafast fiber amplifiers

International Nuclear Information System (INIS)

Hanna, Marc; Guichard, Florent; Druon, Frédéric; Georges, Patrick; Zaouter, Yoann; Papadopoulos, Dimitris N

2016-01-01

We review recent progress in coherent combining of femtosecond pulses amplified in optical fibers as a way to scale the peak and average power of ultrafast sources. Different methods of achieving coherent pulse addition in space (beam combining) and time (divided pulse amplification) domains are described. These architectures can be widely classified into active methods, where the relative phases between pulses are subject to a servomechanism, and passive methods, where phase matching is inherent to the geometry. Other experiments that combine pulses with different spectral contents, pulses that have been nonlinearly broadened or successive pulses from a mode-locked laser oscillator, are then presented. All these techniques allow access to unprecedented parameter range for fiber ultrafast sources. (topical review)

Drilling and the associated drillhole measurements of the pilot hole ONK-PH8

International Nuclear Information System (INIS)

Karttunen, P.; Poellaenen, J.; Rautio, T.; Tarvainen, A.-M.; Lamminmaeki, T.; Kemppainen, K.; Kosunen, P.; Lampinen, H.

2009-02-01

The construction of the ONKALO access tunnel started in September 2004 at Olkiluoto. Most of the investigations related to the construction of the access tunnel aim to ensure successful excavations, reinforcement and sealing. Pilot holes are drillholes, which are core drilled along the tunnel profile. The length of the pilot holes typically varies from several tens of metres to a couple of hundred metres. The pilot holes are aimed to confirm the quality of the rock mass for tunnel construction, and in particular to identify water conductive fractured zones and to provide information that could result in modifications of the existing construction plans. The pilot hole ONK-PH8 was drilled from chainage 3116 to chainage 3266.29 in June- July 2008. The length of the hole is 150.29 metres. The aim during the drilling work was to orient core samples as much as possible. The deviation of the drillhole was measured during and after the drilling phase. Electric conductivity was measured from the collected returning water samples. Water conductivity of the fractures or fractured zones was measured by Posiva Flow Log equipment. The measurements were done in two phases. During flow measurements also grounding resistance, electric conductivity and temperature were measured. In flow logging test sections of 0.5 m and increments of 0.1 m were used. The water loss measurements failed. Logging of the core samples included the following parameters: lithology, foliation, fracturing, fracture frequency, RQD, fractured zones, core loss, and weathering. The rock mechanical logging was based on Q-classification. The test to determine rock strength and deformation were made with Rock Tester-equipment. Geophysical logging and optical imaging of the pilot hole included the fieldwork of all surveys, the integration of the data as well as interpretation of the acoustic and drillhole radar data. One of the objectives of the geochemical study was to get information of the composition of ONKALO

Ultrafast optical signal processing using semiconductor quantum dot amplifiers

DEFF Research Database (Denmark)

Berg, Tommy Winther; Mørk, Jesper

2002-01-01

The linear and nonlinear properties of quantum dot amplifiers are discussed on the basis of an extensive theoretical model. These devices show great potential for linear amplification as well as ultrafast signal processing.......The linear and nonlinear properties of quantum dot amplifiers are discussed on the basis of an extensive theoretical model. These devices show great potential for linear amplification as well as ultrafast signal processing....

Minerals in fractures of the saturated zone from drill core USW G-4, Yucca Mountain, Nye County, Nevada

International Nuclear Information System (INIS)

Carlos, B.A.

1987-04-01

The minerals in fractures in drill core USW G-4, from the static water level (SWL) at 1770 ft to the base of the hole at 3000 ft, were studied to determine their identity and depositional sequence and to compare them with those found above the SWL in the same drill hole. There is no change in mineralogy or mineral morphology across the SWL. The significant change in mineralogy and relationship to the host rock occurs at 1381 ft, well above the present water table. Below 1381 ft clinoptilolite appears in the fractures and rock matrix instead of heulandite, and the fracture mineralogy correlates with the host rock mineralogy. Throughout most of the saturated zone (below the SWL) in USW G-4, zeolites occur in fractures only in zeolitic tuff; however, zeolites persist in fracture below the base of the deepest zeolitic tuff interval. Nonzeolitic intervals of tuff have fewer fractures, and many of these have no coatings; a few have quartz and feldspar coatings. One interval in zeolitic tuff (2125-2140 ft) contains abundant crisobalite coatings in the fractures. Calcite occurs in fractures from 2575 to 2660 ft, usually with the manganese mineral hollandite, and from 2750 to 2765 ft, usually alone. Manganese minerals occur in several intervals. The spatial correlation of zeolites in fractures with zeolitic host rock suggests that both may have been zeolitized at the same time, possibly by water moving laterally through more permeable zones in the tuff. The continuation of zeolites in fractures below the lowest zeolitic interval in this hole suggests that vertical fracture flow may have been important in the deposition of these coatings. Core from deeper intervals in another hole will be examined to determine if that relationship continues. 17 refs., 19 figs

Ultrafast Thermal Transport at Interfaces

Energy Technology Data Exchange (ETDEWEB)

Cahill, David [Univ. of Illinois, Champaign, IL (United States); Murphy, Catherine [Univ. of Illinois, Champaign, IL (United States); Martin, Lane [Univ. of Illinois, Champaign, IL (United States)

2014-10-21

Our research program on Ultrafast Thermal Transport at Interfaces advanced understanding of the mesoscale science of heat conduction. At the length and time scales of atoms and atomic motions, energy is transported by interactions between single-particle and collective excitations. At macroscopic scales, entropy, temperature, and heat are the governing concepts. Key gaps in fundamental knowledge appear at the transitions between these two regimes. The transport of thermal energy at interfaces plays a pivotal role in these scientific issues. Measurements of heat transport with ultrafast time resolution are needed because picoseconds are the fundamental scales where the lack of equilibrium between various thermal excitations becomes a important factor in the transport physics. A critical aspect of our work has been the development of experimental methods and model systems that enabled more precise and sensitive investigations of nanoscale thermal transport.

Testing the blazar sequence and black hole mass scaling with BL Lac objects

NARCIS (Netherlands)

Plotkin, Richard M.; Markoff, Sera; Anderson, Scott F.; Kelly, Brandon C.; Körding, Elmar; Trager, Scott C.; Romero, Gustavo E.; Sunyaev, Rashid A.; Belloni, Tomaso

Jets from accreting black holes appear remarkably similar over eight orders of magnitude in black hole mass, with more massive black holes generally launching more powerful jets. For example, there is an observed correlation, termed the fundamental plane of black hole accretion, between black hole

Testing the blazar sequence and black hole mass scaling with BL Lac objects

NARCIS (Netherlands)

Plotkin, R.M.; Markoff, S.; Anderson, S.F.; Kelly, B.C.; Körding, E.; Trager, S.C.

2010-01-01

Jets from accreting black holes appear remarkably similar over eight orders of magnitude in black hole mass, with more massive black holes generally launching more powerful jets. For example, there is an observed correlation, termed the fundamental plane of black hole accretion, between black hole

Ultrafast optical pump terahertz-probe spectroscopy of strongly correlated electron materials

International Nuclear Information System (INIS)

Averitt, R.D.; Taylor, Antoinette J.; Thorsmolle, V.K.; Jia, Quanxi; Lobad, A.I.; Trugman, S.A.

2001-01-01

We have used optical-pump far-infrared probe spectroscopy to probe the low energy electron dynamics of high temperature superconductors and colossal magnetoresistance manganites. For the superconductor YBa2Cu3O7, picosecond conductivity measurements probe the interplay between Cooper-pairs and quasiparticles. In optimally doped films, the recovery time for long-range phase-coherent pairing increases from ∼1.5 ps at 4K to ∼3.5 ps near Tc, consistent with the closing of the superconducting gap. For underdoped films, the measured recovery time is temperature independent (3.5 ps) in accordance with the presence of a pseudogap. Ultrafast picosecond measurements of optically induced changes in the absolute conductivity of La0:7M0:3MnO3 thin films (M = Ca, Sr) from 10K to ∼0.9Tc reveal a two-component relaxation. A fast, ∼2 ps, conductivity decrease arises from optically induced modification of the effective phonon temperature. The slower component, related to spin-lattice relaxation, has a lifetime that increases upon approaching Tc from below in accordance with an increasing spin specific heat. Our results indicate that for T<< Tc, the conductivity is determined by incoherent phonons while spin fluctuations dominate near Tc.

Inner-shell photoionization and core-hole decay of Xe and XeF2.

Science.gov (United States)

Southworth, Stephen H; Wehlitz, Ralf; Picón, Antonio; Lehmann, C Stefan; Cheng, Lan; Stanton, John F

2015-06-14

Photoionization cross sections and partial ion yields of Xe and XeF2 from Xe 3d(5/2), Xe 3d(3/2), and F 1s subshells in the 660-740 eV range are compared to explore effects of the F ligands. The Xe 3d-ϵf continuum shape resonances dominate the photoionization cross sections of both the atom and molecule, but prominent resonances appear in the XeF2 cross section due to nominal excitation of Xe 3d and F 1s electrons to the lowest unoccupied molecular orbital (LUMO), a delocalized anti-bonding MO. Comparisons of the ion products from the atom and molecule following Xe 3d photoionization show that the charge-state distribution of Xe ions is shifted to lower charge states in the molecule along with production of energetic F(+) and F(2+) ions. This suggests that, in decay of a Xe 3d core hole, charge is redistributed to the F ligands and the system dissociates due to Coulomb repulsion. The ion products from excitation of the F 1s-LUMO resonance are different and show strong increases in the yields of Xe(+) and F(+) ions. The subshell ionization thresholds, the LUMO resonance energies, and their oscillator strengths are calculated by relativistic coupled-cluster methods and agree well with measurements.

Connecting horizon pixels and interior voxels of a black hole

International Nuclear Information System (INIS)

Nicolini, Piero; Singleton, Douglas

2014-01-01

In this paper we discuss to what extent one can infer details of the interior structure of a black hole based on its horizon. Recalling that black hole thermal properties are connected to the non-classical nature of gravity, we circumvent the restrictions of the no-hair theorem by postulating that the black hole interior is singularity free due to violations of the usual energy conditions. Further these conditions allow one to establish a one-to-one, holographic projection between Planckian areal “bits” on the horizon and “voxels”, representing the gravitational degrees of freedom in the black hole interior. We illustrate the repercussions of this idea by discussing an example of the black hole interior consisting of a de Sitter core postulated to arise from the local graviton quantum vacuum energy. It is shown that the black hole entropy can emerge as the statistical entropy of a gas of voxels

Drilling and associated drillhole measurements of the pilot hole ONK-PH11

International Nuclear Information System (INIS)

Karttunen, P.; Mancini, P.; Pekkanen, J.; Poellaenen, J.; Tarvainen, A.-M.; Toropainen, V.; Pere, T.

2011-01-01

The construction of the ONKALO access tunnel started in September 2004 at Olkiluoto. Most of the investigations related to the construction of the access tunnel aim to ensure successful excavations, reinforcement and sealing. Pilot holes are drillholes, which are core drilled along the tunnel profile. The length of the pilot holes typically varies from several tens of metres to a couple of hundred metres. The pilot holes are aimed to confirm the quality of the rock mass for tunnel construction, and in particular to identify water conductive fractured zones and to provide information that could result in modifications of the existing construction plans. The pilot hole ONK-PH11 was drilled from chainage 3922 to chainage 4053 in October 2009. The length of the hole is 131.21 metres. The aim during the drilling work was to orient core samples as much as possible. The deviation of the drillhole was measured during and after the drilling phase. Electric conductivity was measured from the collected returning water samples. Hydraulic conductivity of the fractures or fractured zones was measured by Posiva Flow Log equipment. During flow measurements also electric conductivity and temperature were measured. In flow logging test sections of 0.5 m and increments of 0.1 m were used. The water loss measurements were performed after drilling was completed by the drilling company. Logging of the core samples included the following parameters: lithology, foliation, fracturing, RQD, fractured zones, weathering and possible intersections. The rock mechanical logging was based on Q-classification. The rock strength and deformation were determined with Rock Tester -equipment. Geophysical logging and optical imaging of the pilot hole included the fieldwork of all surveys, the integration of the data as well as interpretation of the acoustic and drillhole radar data. The groundwater samples were collected from the open hole without any packers. The collected groundwater samples were

Strong deflection gravitational lensing by a modified Hayward black hole

Energy Technology Data Exchange (ETDEWEB)

Zhao, Shan-Shan; Xie, Yi [Nanjing University, School of Astronomy and Space Science, Nanjing (China); Nanjing University, Ministry of Education, Key Laboratory of Modern Astronomy and Astrophysics, Nanjing (China)

2017-05-15

A modified Hayward black hole is a nonsingular black hole. It is proposed that it would form when the pressure generated by quantum gravity can stop matter's collapse as the matter reaches the Planck density. Strong deflection gravitational lensing occurring nearby its event horizon might provide some clues of these quantum effects in its central core. We investigate observables of the strong deflection lensing, including angular separations, brightness differences and time delays between its relativistic images, and we estimate their values for the supermassive black hole in the Galactic center. We find that it is possible to distinguish the modified Hayward black hole from a Schwarzschild one, but it demands a very high resolution, beyond current stage. (orig.)

Ultrafast vibrations of gold nanorings

DEFF Research Database (Denmark)

Kelf, T; Tanaka, Y; Matsuda, O

2011-01-01

We investigate the vibrational modes of gold nanorings on a silica substrate with an ultrafast optical technique. By comparison with numerical simulations, we identify several resonances in the gigahertz range associated with axially symmetric deformations of the nanoring and substrate. We...

Ultrafast control and monitoring of material properties using terahertz pulses

Energy Technology Data Exchange (ETDEWEB)

Bowlan, Pamela Renee [Los Alamos National Lab. (LANL), Los Alamos, NM (United States). Lab. for Ultrafast Materials Optical Science (LUMOS)

2016-05-02

These are a set of slides on ultrafast control and monitoring of material properties using terahertz pulses. A few of the topics covered in these slides are: How fast is a femtosecond (fs), Different frequencies probe different properties of molecules or solids, What can a THz pulse do to a material, Ultrafast spectroscopy, Generating and measuring ultrashort THz pulses, Tracking ultrafast spin dynamics in antiferromagnets through spin wave resonances, Coherent two-dimensional THz spectroscopy, and Probing vibrational dynamics at a surface. Conclusions are: Coherent two-dimensional THz spectroscopy: a powerful approach for studying coherence and dynamics of low energy resonances. Applying this to graphene we investigated the very strong THz light mater interaction which dominates over scattering. Useful for studying coupled excitations in multiferroics and monitoring chemical reactions. Also, THz-pump, SHG-probe spectoscopy: an ultrafast, surface sensitive probe of atomic-scale symmetry changes and nonlinear phonon dymanics. We are using this in Bi₂Se₃ to investigate the nonlinear surface phonon dynamics. This is potentially very useful for studying catalysis.

Electrically-driven GHz range ultrafast graphene light emitter (Conference Presentation)

Science.gov (United States)

Kim, Youngduck; Gao, Yuanda; Shiue, Ren-Jye; Wang, Lei; Aslan, Ozgur Burak; Kim, Hyungsik; Nemilentsau, Andrei M.; Low, Tony; Taniguchi, Takashi; Watanabe, Kenji; Bae, Myung-Ho; Heinz, Tony F.; Englund, Dirk R.; Hone, James

2017-02-01

Ultrafast electrically driven light emitter is a critical component in the development of the high bandwidth free-space and on-chip optical communications. Traditional semiconductor based light sources for integration to photonic platform have therefore been heavily studied over the past decades. However, there are still challenges such as absence of monolithic on-chip light sources with high bandwidth density, large-scale integration, low-cost, small foot print, and complementary metal-oxide-semiconductor (CMOS) technology compatibility. Here, we demonstrate the first electrically driven ultrafast graphene light emitter that operate up to 10 GHz bandwidth and broadband range (400 1600 nm), which are possible due to the strong coupling of charge carriers in graphene and surface optical phonons in hBN allow the ultrafast energy and heat transfer. In addition, incorporation of atomically thin hexagonal boron nitride (hBN) encapsulation layers enable the stable and practical high performance even under the ambient condition. Therefore, electrically driven ultrafast graphene light emitters paves the way towards the realization of ultrahigh bandwidth density photonic integrated circuits and efficient optical communications networks.

Supermassive Black Holes in Active Galactic Nuclei. II. Calibration of the Black Hole Mass-Velocity Dispersion Relationship for Active Galactic Nuclei

DEFF Research Database (Denmark)

Onken, Christopher A.; Ferrarese, Laura; Merritt, David

2004-01-01

We calibrate reverberation-based black hole masses in active galactic nuclei (AGNs) by using the correlation between black hole mass, M, and bulge/spheroid stellar velocity dispersion, sigma. We use new measurements of sigma for 6 AGNs and published velocity dispersions for 10 others......, in conjunction with improved reverberation mapping results, to determine the scaling factor required to bring reverberation-based black hole masses into agreement with the quiescent galaxy M-sigma relationship. The scatter in the AGN black hole masses is found to be less than a factor of 3. The current...

Ultrafast demagnetisation dependence on film thickness: A TDDFT calculation

Science.gov (United States)

Singh, N.; Sharma, S.

2018-04-01

Ferromagnetic materials when subjected to intense laser pulses leads to reduction of their magnetisation on an ultrafast scale. Here, we perform an ab-initio calculation to study the behavior of ultrafast demagnetisation as a function of film thickness for Nickel as compared to the bulk of the material. In thin films surface formation results in amplification of demagnetisation with the percentage of demagnetisation depending upon the film thickness.

Drilling and associated drillhole measurements of the pilot hole ONK-PH12

International Nuclear Information System (INIS)

Toropainen, V.; Tarvainen, A.-M.; Poellaenen, J.; Pekkanen, J.; Pere, T.; Kaepyaho, E.; Lahti, M.

2011-01-01

The construction of the ONKALO access tunnel started in September 2004 at Olkiluoto. Most of the investigations related to the construction of the access tunnel aim to ensure successful excavations, reinforcement and sealing. Pilot holes are drillholes, which are core drilled along the tunnel profile. The length of the pilot holes typically varies from several tens of metres to a couple of hundred metres. The pilot holes are aimed to confirm the quality of the rock mass for tunnel construction, and in particular to identify water conductive fractured zones and to provide information that could result in modifications of the existing construction plans. The pilot hole ONK-PH12 was drilled from ONKALO chainage 4092 to chainage 4215 in January 2010. The length of the hole is 123.96 metres. The drilling method was orientated core drilling. The deviation of the drillhole was measured during and after the drilling phase. Electric conductivity was measured from the collected returning water samples. Logging of the core samples included the following parameters: lithology, foliation, fracturing, fracture frequency, RQD, fractured zones, core loss, and weathering. The rock mechanical logging was based on Q-classification. The test to determine rock strength and deformation were made with Rock Tester -equipment. Water conductivity of the fractures or fractured zones was measured by Posiva Flow Log equipment. The measurements were done in two phases. During flow measurements also grounding resistance electric conductivity and temperature were measured. In flow logging test, sections of 0.5 m with increments of 0.1 m were used. Water loss measurements were conducted in the drillhole section 5.0-123.85 m dhd. Geophysical logging as well as optical and acoustic imaging of the pilot hole included the fieldwork of all surveys, the integration of the data as well as interpretation of the acoustic and drillhole radar data. Groundwater sampling was not applicable because no

Influence of Steel Reinforcement on In-Situ Stress Evaluation in Concrete Structures by the Core-Drilling Method

International Nuclear Information System (INIS)

McGinnis, M. J.; Pessiki, S.

2006-01-01

The core-drilling method is an emerging technique for evaluating in-situ stress in a concrete structure. A small hole is drilled into the structure, and the deformations in the vicinity of the hole are measured and related via elasticity theory to the stress. The method is similar to the ASTM hole-drilling strain-gauge method excepting that displacements rather than strains are the measured quantities. The technique may be considered nondestructive since the ability of the structure to perform its function is unaffected, and the hole is easily repaired. Displacement measurements in the current work are performed using 3D digital image correlation and industrial photogrammetry. The current paper addresses perturbations in the method caused by steel reinforcement within the concrete. The reinforcement is significantly stiffer than the surrounding concrete, altering the expected displacement field. A numerical investigation performed indicates an under-prediction of stress by as much as 18 percent in a heavily reinforced structure, although the effect is significantly smaller for more common amounts of reinforcement

Influence of Steel Reinforcement on In-Situ Stress Evaluation in Concrete Structures by the Core-Drilling Method

Science.gov (United States)

McGinnis, M. J.; Pessiki, S.

2006-03-01

The core-drilling method is an emerging technique for evaluating in-situ stress in a concrete structure. A small hole is drilled into the structure, and the deformations in the vicinity of the hole are measured and related via elasticity theory to the stress. The method is similar to the ASTM hole-drilling strain-gauge method excepting that displacements rather than strains are the measured quantities. The technique may be considered nondestructive since the ability of the structure to perform its function is unaffected, and the hole is easily repaired. Displacement measurements in the current work are performed using 3D digital image correlation and industrial photogrammetry. The current paper addresses perturbations in the method caused by steel reinforcement within the concrete. The reinforcement is significantly stiffer than the surrounding concrete, altering the expected displacement field. A numerical investigation performed indicates an under-prediction of stress by as much as 18 percent in a heavily reinforced structure, although the effect is significantly smaller for more common amounts of reinforcement.

Ultrafast Exciton Dissociation and Long-Lived Charge Separation in a Photovoltaic Pentacene-MoS2 van der Waals Heterojunction.

Science.gov (United States)

Bettis Homan, Stephanie; Sangwan, Vinod K; Balla, Itamar; Bergeron, Hadallia; Weiss, Emily A; Hersam, Mark C

2017-01-11

van der Waals heterojunctions between two-dimensional (2D) layered materials and nanomaterials of different dimensions present unique opportunities for gate-tunable optoelectronic devices. Mixed-dimensional p-n heterojunction diodes, such as p-type pentacene (0D) and n-type monolayer MoS 2 (2D), are especially interesting for photovoltaic applications where the absorption cross-section and charge transfer processes can be tailored by rational selection from the vast library of organic molecules and 2D materials. Here, we study the kinetics of excited carriers in pentacene-MoS 2 p-n type-II heterojunctions by transient absorption spectroscopy. These measurements show that the dissociation of MoS 2 excitons occurs by hole transfer to pentacene on the time scale of 6.7 ps. In addition, the charge-separated state lives for 5.1 ns, up to an order of magnitude longer than the recombination lifetimes from previously reported 2D material heterojunctions. By studying the fractional amplitudes of the MoS 2 decay processes, the hole transfer yield from MoS 2 to pentacene is found to be ∼50%, with the remaining holes undergoing trapping due to surface defects. Overall, the ultrafast charge transfer and long-lived charge-separated state in pentacene-MoS 2 p-n heterojunctions suggest significant promise for mixed-dimensional van der Waals heterostructures in photovoltaics, photodetectors, and related optoelectronic technologies.

Ultrafast magnetodynamics with free-electron lasers

Science.gov (United States)

Malvestuto, Marco; Ciprian, Roberta; Caretta, Antonio; Casarin, Barbara; Parmigiani, Fulvio

2018-02-01

The study of ultrafast magnetodynamics has entered a new era thanks to the groundbreaking technological advances in free-electron laser (FEL) light sources. The advent of these light sources has made possible unprecedented experimental schemes for time-resolved x-ray magneto-optic spectroscopies, which are now paving the road for exploring the ultimate limits of out-of-equilibrium magnetic phenomena. In particular, these studies will provide insights into elementary mechanisms governing spin and orbital dynamics, therefore contributing to the development of ultrafast devices for relevant magnetic technologies. This topical review focuses on recent advancement in the study of non-equilibrium magnetic phenomena from the perspective of time-resolved extreme ultra violet (EUV) and soft x-ray spectroscopies at FELs with highlights of some important experimental results.

Femtochemistry and femtobiology ultrafast dynamics in molecular science

CERN Document Server

Douhal, Abderrazzak

2002-01-01

This book contains important contributions from top international scientists on the-state-of-the-art of femtochemistry and femtobiology at the beginning of the new millennium. It consists of reviews and papers on ultrafast dynamics in molecular science.The coverage of topics highlights several important features of molecular science from the viewpoint of structure (space domain) and dynamics (time domain). First of all, the book presents the latest developments, such as experimental techniques for understanding ultrafast processes in gas, condensed and complex systems, including biological mol

Growth of black holes in the interior of rotating neutron stars

DEFF Research Database (Denmark)

Kouvaris, C.; Tinyakov, P.

2014-01-01

Mini-black holes made of dark matter that can potentially form in the interior of neutron stars always have been thought to grow by accreting the matter of the core of the star via a spherical Bondi accretion. However, neutron stars have sometimes significant angular velocities that can...... in principle stall the spherical accretion and potentially change the conclusions derived about the time it takes for black holes to destroy a star. We study the effect of the star rotation on the growth of such black holes and the evolution of the black hole spin. Assuming no mechanisms of angular momentum...... evacuation, we find that even moderate rotation rates can in fact destroy spherical accretion at the early stages of the black hole growth. However, we demonstrate that the viscosity of nuclear matter can alleviate the effect of rotation, making it possible for the black hole to maintain spherical accretion...

Ultrafast spectroscopy of biological photoreceptors

NARCIS (Netherlands)

Kennis, J.T.M.; Groot, M.L.

2007-01-01

We review recent new insights on reaction dynamics of photoreceptors proteins gained from ultrafast spectroscopy. In Blue Light sensing Using FAD (BLUF) domains, a hydrogen-bond rearrangement around the flavin chromophore proceeds through a radical-pair mechanism, by which light-induced electron and

Ultrafast vibrations of gold nanorings

DEFF Research Database (Denmark)

Kelf, T; Tanaka, Y; Matsuda, O

2011-01-01

We investigate the vibrational modes of gold nanorings on a silica substrate with an ultrafast optical technique. By comparison with numerical simulations, we identify several resonances in the gigahertz range associated with axially symmetric deformations of the nanoring and substrate. We elucid...

Drilling and associated drillhole measurements of the pilot hole ONK-PH13

International Nuclear Information System (INIS)

Tarvainen, A.-M.; Toropainen, V.; Pekkanen, J.; Poellaenen, J.; Kosunen, P.; Lahti, M.; Pere, T.; Aalto, P.

2011-04-01

The construction of ONKALO access tunnel started in September 2004 at Olkiluoto. During the construction, investigations serving both research and construction purposes need to be done. Investigations can be done for example in so called pilot holes. Pilot holes are cored drillholes to be drilled to the tunnel profile. The length of the holes varies from some tens of meters to some hundreds of meters. The purpose of the holes is to confirm the quality of the rock mass for tunnel construction, especially to identify water conductive fractures/fracture zones and provide information that could result in modifications of the existing construction plans. The pilot hole ONK-KR13 was drilled in March 2010. Drilling was started from chainage 4201. The final length of the hole was 140.05 meters. The deviation of the drillhole was measured during and after the drilling. Additionally, oriented core samples were collected and electric conductivity of returning water from the drill hole was measured. Logging of the core samples included following parameters: lithology, foliation, fracturing, fracture frequency, RQD, fractured zones, core loss and weathering. The rock mechanical logging was based on Q-classification. The strength and deformation properties of the rock were defined by using Rock-Tester equipment. Hydraulic measurements were made by using the PFL DIFF (Posiva Flow Log, Difference Flow method). PFL DIFF measurements were performed with a 0.5 m section length and with 0.1 m length increments. With PFL DIFF tool the locations of flowing fractures and their transmissivities were detected. Simultaneously, the electric conductivity (EC) of the drillhole water and fracture-specific water, temperature of the drillhole water, single point resistance (SPR) of the drillhole wall and the prevailing water pressure profile were measured. Water loss measurements were done after the drilling by the tool developed by Posiva. The equipment was in test use during the measurements

Ultrafast surface-enhanced Raman spectroscopy.

Science.gov (United States)

Keller, Emily L; Brandt, Nathaniel C; Cassabaum, Alyssa A; Frontiera, Renee R

2015-08-07

Ultrafast surface-enhanced Raman spectroscopy (SERS) with pico- and femtosecond time resolution has the ability to elucidate the mechanisms by which plasmons mediate chemical reactions. Here we review three important technological advances in these new methodologies, and discuss their prospects for applications in areas including plasmon-induced chemistry and sensing at very low limits of detection. Surface enhancement, arising from plasmonic materials, has been successfully incorporated with stimulated Raman techniques such as femtosecond stimulated Raman spectroscopy (FSRS) and coherent anti-Stokes Raman spectroscopy (CARS). These techniques are capable of time-resolved measurement on the femtosecond and picosecond time scale and can be used to follow the dynamics of molecules reacting near plasmonic surfaces. We discuss the potential application of ultrafast SERS techniques to probe plasmon-mediated processes, such as H2 dissociation and solar steam production. Additionally, we discuss the possibilities for high sensitivity SERS sensing using these stimulated Raman spectroscopies.

Critical Phenomena in Higher Curvature Charged AdS Black Holes

Directory of Open Access Journals (Sweden)

Arindam Lala

2013-01-01

Full Text Available In this paper, we have studied the critical phenomena in higher curvature charged AdS black holes. We have considered Lovelock-Born-Infeld-AdS black hole as an example. The thermodynamics of the black hole have been studied which reveals the onset of a higher-order phase transition in the black hole in the canonical ensemble (fixed charge ensemble framework. We have analytically derived the critical exponents associated with these thermodynamic quantities. We find that our results fit well with the thermodynamic scaling laws and consistent with the mean field theory approximation. The suggestive values of the other two critical exponents associated with the correlation function and correlation length on the critical surface have been derived.

Ultrafast Infrared and UV-vis Studies of the Photochemistry of Methoxycarbonylphenyl Azides in Solution

OpenAIRE

Xue, Jiadan; Luk, Hoi Ling; Eswaran, S. V.; Hadad, Christopher M.; Platz, Matthew S.

2012-01-01

The photochemistry of 4-methoxycarbonylphenyl azide (2a), 2-methoxycarbonylphenyl azide (3a) and 2-methoxy-6-methoxycarbonylphenyl azide (4a) were studied by ultrafast time-resolved infrared (IR) and UV-vis spectroscopies in solution. Singlet nitrenes and ketenimines were observed and characterized for all three azides. Isoxazole species 3g and 4g are generated after photolysis of 3a and 4a, respectively, in acetonitrile. Triplet nitrene 4e formation correlated with the decay of singlet nitre...

Ultrafast gas switching experiments

International Nuclear Information System (INIS)

Frost, C.A.; Martin, T.H.; Patterson, P.E.; Rinehart, L.F.; Rohwein, G.J.; Roose, L.D.; Aurand, J.F.; Buttram, M.T.

1993-01-01

We describe recent experiments which studied the physics of ultrafast gas breakdown under the extreme overvoltages which occur when a high pressure gas switch is pulse charged to hundreds of kV in 1 ns or less. The highly overvolted peaking gaps produce powerful electromagnetic pulses with risetimes Khz at > 100 kV/m E field

Clinico-morphological correlations in the categorization of holes between the ventricles

Directory of Open Access Journals (Sweden)

Friedman Brad

2010-01-01

Full Text Available Controversy still exists in the categorization of holes between the ventricles, although they are the most common congenital cardiac malformation. Advanced imaging techniques such as three-dimensional echocardiography and computed tomographic angiography offer superb anatomical details of these defects. In this review, we have sought to collate the features highlighted in different categorizations and identify their similarities, but also emphasize their differences. We hope that an analysis of this type, now achievable during life, using advanced imaging, might lead to the appearance of a unified system for diagnosis and description of holes between the ventricles.

The correlation of coal beds in Squaw Basin and part of Eden Ridge, T. 33 S., R. 11 W., W. M., southwestern Oregon

Science.gov (United States)

Wayland, Russell Gibson

1965-01-01

A conflict in correlation of coal beds dating from 1914 is reexamined-with the aid of new. core hole data, photogeologic interpretation, a broader understanding of the stratigraphy, and brief field studies. It is concluded that the known coal beds in Squaw Basin area of limited lateral extent and are older than those exposed at Eden Ridge. Similar coal beds may be found in other rocks of the Tyee Formation in this area. More core drilling could be justified.

Back up core designs for the experimental multi-purpose VHTR

International Nuclear Information System (INIS)

Aochi, Tetsuo; Yasuno, Takehiko; Miyamoto, Yoshiaki; Shindo, Ryuichi; Ikushima, Takeshi

1979-02-01

For the Experimental Multi-Purpose Very High Temperature Reactor (thermal power 50 MW and reactor outlet helium temperature 1000 0 C), design studies have been made of two backup cores loaded with new-type fuel elements. The purpose is to improve core operational characteristics, especially in thermohydraulics, of the reference design core consisting of pin-in-block type fuel elements having externally cooled hollow fuel rods. In this report are described the design principles and the analyses made of nuclear, thermal and hydraulic, fuel, and safety performances to determine the backup fuel and core design parameters. The first backup core (SP fuel core) is composed of fuel elements with internally cooled fuel rods (semi-pin), 36 rods in each standard element and 18 rods in each control element. The second backup core (MH fuel core) is composed of multihole fuel elements. 102 fuel and 54 coolant holes in each standard element and 30 fuel and 18 coolant holes in each control element. Either of the cores has 73 fuel columns 4 m high; the arrangement of active core and reactor internal structures is the same as that in the reference design. The backup cores meet nearly all design requirements of the VHTR, permitting the rated power operation with coolant Reynolds number of over 10,000 in the SP core and over 6,000 in the MH core. (author)

Ultrafast spin exchange-coupling torque via photo-excited charge-transfer processes

Science.gov (United States)

Ma, X.; Fang, F.; Li, Q.; Zhu, J.; Yang, Y.; Wu, Y. Z.; Zhao, H. B.; Lüpke, G.

2015-10-01

Optical control of spin is of central importance in the research of ultrafast spintronic devices utilizing spin dynamics at short time scales. Recently developed optical approaches such as ultrafast demagnetization, spin-transfer and spin-orbit torques open new pathways to manipulate spin through its interaction with photon, orbit, charge or phonon. However, these processes are limited by either the long thermal recovery time or the low-temperature requirement. Here we experimentally demonstrate ultrafast coherent spin precession via optical charge-transfer processes in the exchange-coupled Fe/CoO system at room temperature. The efficiency of spin precession excitation is significantly higher and the recovery time of the exchange-coupling torque is much shorter than for the demagnetization procedure, which is desirable for fast switching. The exchange coupling is a key issue in spin valves and tunnelling junctions, and hence our findings will help promote the development of exchange-coupled device concepts for ultrafast coherent spin manipulation.

The Extragalactic Lens VLBI Imaging Survey (ELVIS): Investigating galaxy cores and black holes with gravitational lens central images

Science.gov (United States)

Boyce, Edward R.

This thesis describes the Extragalactic Lens VLBI Imaging Survey (ELVIS), a search for central images in gravitational lenses. We present the first four ELVIS targets, for which we have radio VLBI observations with resolutions of a few milli-arcseconds and sensitivities of 15 - 38mJy. For PMN J1838-3427, CLASS B0739+366 and CLASS B0445+123 we have not detected any central images, but have set stringent upper limits on their flux densities. For CLASS B2319+051 we have made a tentative detection of a third radio source, which may be either a central image or radio emission from the lens galaxy. Using the upper limits on the central image flux densities, we gain new information about the matter distributions in the lens galaxies of these systems. We fit a broken power law model for the matter profile, and constrain the allowed break radii and inner index of this model. To demagnify the central images to the observed level the matter profiles must be slightly shallower than or steeper than isothermal, which is consistent with previous studies of early type galaxy profiles. The presence of a super-massive black hole weakens the constraints somewhat, but the profiles are still close to isothermal. Relative to previous work, we reduce the maximum sizes of shallow cores by factors of 2 to 3, and raise the indices of r 0( r -g central cusps by g = 0.05 - 0.35. If we take the source in B2319+051 to be a central image, then we select a narrow band of allowed break radii and inner indices, finding that a constant density core has size 150--380 pc, and a pure power law has index g = 1.5 - 1.67. Our constraints still allow sufficiently shallow profiles that some super-massive black holes may form central image pairs rather than eliminating the central image, and these image pairs may be detected with future instruments. (Copies available exclusively from MIT Libraries, Rm. 14-0551, Cambridge, MA 02139-4307. Ph. 617-253-5668; Fax 617-253-1690.)

Ultrafast magnetization dynamics

OpenAIRE

Woodford, Simon

2008-01-01

This thesis addresses ultrafast magnetization dynamics from a theoretical perspective. The manipulation of magnetization using the inverse Faraday effect has been studied, as well as magnetic relaxation processes in quantum dots. The inverse Faraday effect – the generation of a magnetic field by nonresonant, circularly polarized light – offers the possibility to control and reverse magnetization on a timescale of a few hundred femtoseconds. This is important both for the technological advant...

Tissue strain rate estimator using ultrafast IQ complex data

OpenAIRE

TERNIFI , Redouane; Elkateb Hachemi , Melouka; Remenieras , Jean-Pierre

2012-01-01

International audience; Pulsatile motion of brain parenchyma results from cardiac and breathing cycles. In this study, transient motion of brain tissue was estimated using an Aixplorer® imaging system allowing an ultrafast 2D acquisition mode. The strain was computed directly from the ultrafast IQ complex data using the extended autocorrelation strain estimator (EASE), which provides great SNRs regardless of depth. The EASE first evaluates the autocorrelation function at each depth over a set...

ULTRAMASSIVE BLACK HOLE COALESCENCE

International Nuclear Information System (INIS)

Khan, Fazeel Mahmood; Holley-Bockelmann, Kelly; Berczik, Peter

2015-01-01

Although supermassive black holes (SMBHs) correlate well with their host galaxies, there is an emerging view that outliers exist. Henize 2-10, NGC 4889, and NGC 1277 are examples of SMBHs at least an order of magnitude more massive than their host galaxy suggests. The dynamical effects of such ultramassive central black holes is unclear. Here, we perform direct N-body simulations of mergers of galactic nuclei where one black hole is ultramassive to study the evolution of the remnant and the black hole dynamics in this extreme regime. We find that the merger remnant is axisymmetric near the center, while near the large SMBH influence radius, the galaxy is triaxial. The SMBH separation shrinks rapidly due to dynamical friction, and quickly forms a binary black hole; if we scale our model to the most massive estimate for the NGC 1277 black hole, for example, the timescale for the SMBH separation to shrink from nearly a kiloparsec to less than a parsec is roughly 10 Myr. By the time the SMBHs form a hard binary, gravitational wave emission dominates, and the black holes coalesce in a mere few Myr. Curiously, these extremely massive binaries appear to nearly bypass the three-body scattering evolutionary phase. Our study suggests that in this extreme case, SMBH coalescence is governed by dynamical friction followed nearly directly by gravitational wave emission, resulting in a rapid and efficient SMBH coalescence timescale. We discuss the implications for gravitational wave event rates and hypervelocity star production

Characterization of Nanostructured Semiconductors by Ultrafast Luminescence Imaging

Science.gov (United States)

Blake, Jolie

-diffusion controlled recombination. In the second phase of this study the setup was configured to the ultraviolet detection range for measuring the nanowires of conductive metal oxides. ZnO was the metal oxide of focus in this research. Ultrafast measurements were conducted on ZnO nanowires and ASE dynamics from multiple regions along a nanowire were again fitted to the ASE model and the recombination constants extracted. The diminished influence of the Shockley-Read-Hall recombination rate on the measured luminescence suggested that leading quadratic term in the model is a measure of a two-body defect mediated recombination rate, from which a defect density could be calculated. The measured change in defect density along the length of the nanowire correlated with changes in the growth conditions that established a defect gradient. The results show that the Kerr-gated system, as well as being a probe of ultrafast dynamics, is also a new tool for measuring changes in defect density in single nanostructures.

Overview of Hole GT2A: Drilling middle gabbro in Wadi Tayin massif, Oman ophiolite

Science.gov (United States)

Takazawa, E.; Kelemen, P. B.; Teagle, D. A. H.; Coggon, J. A.; Harris, M.; Matter, J. M.; Michibayashi, K.

2017-12-01

Hole GT2A (UTM: 40Q 655960.7E / 2529193.5N) was drilled by the Oman Drilling Project (OmDP) into Wadi Gideah of Wadi Tayin massif in the Samail ophiolite, Oman. OmDP is an international collaboration supported by the International Continental Scientific Drilling Program, the Deep Carbon Observatory, NSF, IODP, JAMSTEC, and the European, Japanese, German and Swiss Science Foundations, with in-kind support in Oman from the Ministry of Regional Municipalities and Water Resources, Public Authority of Mining, Sultan Qaboos University, and the German University of Technology. Hole GT2A was diamond cored in 25 Dec 2016 to 18 Jan 2017 to a total depth of 406.77 m. The outer surfaces of the cores were imaged and described on site before being curated, boxed and shipped to the IODP drill ship Chikyu, where they underwent comprehensive visual and instrumental analysis. 33 shipboard scientists were divided into six teams (Igneous, Alteration, Structural, Geochem, Physical Properties, Paleomag) to describe and analyze the cores. Hole GT2A drilled through the transition between foliated and layered gabbro. The transition zone occurs between 50 and 150 m curation corrected depth (CCD). The top 50 m of Hole GT2A is foliated gabbro whereas the bottom 250 m consists of layered gabbro. Brittle fracture is observed throughout the core. Intensity of alteration vein decreases from the top to the bottom of the hole. On the basis of changes in grain size and/or modal abundance and/or appearance/disappearance of igneous primary mineral(s) five lithological units are defined in Hole GT2A (Unit I to V). The uppermost part of Hole GT2A (Unit I) is dominated by fine-grained granular olivine gabbro intercalated with less dominant medium-grained granular olivine gabbro and rare coarse-grained varitextured gabbro. The lower part of the Hole (Units II, III and V) is dominated by medium-grained olivine gabbro, olivine melagabbro and olivine-bearing gabbro. Modally-graded rhythmic layering with

Patellofemoral joint motion: Evaluation by ultrafast computed tomography

International Nuclear Information System (INIS)

Stanford, W.; Phelan, J.; Kathol, M.H.; Rooholamini, S.A.; El-Khoury, G.Y.; Palutsis, G.R.; Albright, J.P.

1988-01-01

Patellofemoral maltracking is a recognized cause of peripatellar pain. Clinicians currently rely on observation, palpation, and static radiographic images to evaluate the symptomatic patient. Ultrafast computed tomography (ultrafast CT) offers objective observations of the dynamic influences of muscle contraction on the patellofemoral joint as the knee is actively moved through a range of motion from 90 0 C flexion of full extension. This study reports our initial observations and establishes a range of normal values so that patients with a clinical suspicion of patellar maltracking may be evaluated. (orig./GDG)

Patellofemoral joint motion: Evaluation by ultrafast computed tomography

Energy Technology Data Exchange (ETDEWEB)

Stanford, W.; Phelan, J.; Kathol, M.H.; Rooholamini, S.A.; El-Khoury, G.Y.; Palutsis, G.R.; Albright, J.P.

1988-10-01

Patellofemoral maltracking is a recognized cause of peripatellar pain. Clinicians currently rely on observation, palpation, and static radiographic images to evaluate the symptomatic patient. Ultrafast computed tomography (ultrafast CT) offers objective observations of the dynamic influences of muscle contraction on the patellofemoral joint as the knee is actively moved through a range of motion from 90/sup 0/C flexion of full extension. This study reports our initial observations and establishes a range of normal values so that patients with a clinical suspicion of patellar maltracking may be evaluated. (orig./GDG).

Major and trace elements in Mahogany zone oil shale in two cores from the Green River Formation, piceance basin, Colorado

Science.gov (United States)

Tuttle, M.L.; Dean, W.E.; Parduhn, N.L.

1983-01-01

The Parachute Creek Member of the lacustrine Green River Formation contains thick sequences of rich oil-shale. The richest sequence and the richest oil-shale bed occurring in the member are called the Mahogany zone and the Mahogany bed, respectively, and were deposited in ancient Lake Uinta. The name "Mahogany" is derived from the red-brown color imparted to the rock by its rich-kerogen content. Geochemical abundance and distribution of eight major and 18 trace elements were determined in the Mahogany zone sampled from two cores, U. S. Geological Survey core hole CR-2 and U. S. Bureau of Mines core hole O1-A (Figure 1). The oil shale from core hole CR-2 was deposited nearer the margin of Lake Uinta than oil shale from core hole O1-A. The major- and trace-element chemistry of the Mahogany zone from each of these two cores is compared using elemental abundances and Q-mode factor modeling. The results of chemical analyses of 44 CR-2 Mahogany samples and 76 O1-A Mahogany samples are summarized in Figure 2. The average geochemical abundances for shale (1) and black shale (2) are also plotted on Figure 2 for comparison. The elemental abundances in the samples from the two cores are similar for the majority of elements. Differences at the 95% probability level are higher concentrations of Ca, Cu, La, Ni, Sc and Zr in the samples from core hole CR-2 compared to samples from core hole O1-A and higher concentrations of As and Sr in samples from core hole O1-A compared to samples from core hole CR-2. These differences presumably reflect slight differences in depositional conditions or source material at the two sites. The Mahogany oil shale from the two cores has lower concentrations of most trace metals and higher concentrations of carbonate-related elements (Ca, Mg, Sr and Na) compared to the average shale and black shale. During deposition of the Mahogany oil shale, large quantities of carbonates were precipitated resulting in the enrichment of carbonate-related elements

Real-Space Imaging of Carrier Dynamics of Materials Surfaces by Second-Generation Four-Dimensional Scanning Ultrafast Electron Microscopy

KAUST Repository

Sun, Jingya

2015-09-14

In the fields of photocatalysis and photovoltaics, ultrafast dynamical processes, including carrier trapping and recombination on material surfaces, are among the key factors that determine the overall energy conversion efficiency. A precise knowledge of these dynamical events on the nanometer (nm) and femtosecond (fs) scales was not accessible until recently. The only way to access such fundamental processes fully is to map the surface dynamics selectively in real space and time. In this study, we establish a second generation of four-dimensional scanning ultrafast electron microscopy (4D S-UEM) and demonstrate the ability to record time-resolved images (snapshots) of material surfaces with 650 fs and ∼5 nm temporal and spatial resolutions, respectively. In this method, the surface of a specimen is excited by a clocking optical pulse and imaged using a pulsed primary electron beam as a probe pulse, generating secondary electrons (SEs), which are emitted from the surface of the specimen in a manner that is sensitive to the local electron/hole density. This method provides direct and controllable information regarding surface dynamics. We clearly demonstrate how the surface morphology, grains, defects, and nanostructured features can significantly impact the overall dynamical processes on the surface of photoactive-materials. In addition, the ability to access two regimes of dynamical probing in a single experiment and the energy loss of SEs in semiconductor-nanoscale materials will also be discussed.

Reduction of coupling loss to photonic crystal fibers by controlled hole collapse: A numerical study

DEFF Research Database (Denmark)

Lægsgaard, Jesper; Bjarklev, Anders Overgaard

2004-01-01

The mode profile evolution of small-core photonic crystal fibers (PCFs) during a gradual collapse of the cladding airholes is investigated. The mode overlap with standard step-index fibers having a small index contrast is calculated, and it is found that overlaps around 90% can be achieved in all...... cases studied, with the proper degree of hole collapse. Thus, hole collapse induced by, e.g. laser irradiation could prove an efficient and practical way of reducing splice losses when coupling small-core PCFs to other fiber types....

Mode-coupling in photonic crystal fibers with multiple cores

DEFF Research Database (Denmark)

Kristensen, Martin

2000-01-01

Summary form only given. We have fabricated a photonic crystal fiber (PCF) with multiple cores by drawing a fiber preform from stacked glass tubes. Transmission is high through each core despite many unintentional defects in the cladding indicating that the guidance is determined by the holes near...

Deconvolving instrumental and intrinsic broadening in core-shell x-ray spectroscopies

International Nuclear Information System (INIS)

Fister, T. T.; Seidler, G. T.; Rehr, J. J.; Kas, J. J.; Nagle, K. P.; Elam, W. T.; Cross, J. O.

2007-01-01

Intrinsic and experimental mechanisms frequently lead to broadening of spectral features in core-shell spectroscopies. For example, intrinsic broadening occurs in x-ray absorption spectroscopy (XAS) measurements of heavy elements where the core-hole lifetime is very short. On the other hand, nonresonant x-ray Raman scattering (XRS) and other energy loss measurements are more limited by instrumental resolution. Here, we demonstrate that the Richardson-Lucy (RL) iterative algorithm provides a robust method for deconvolving instrumental and intrinsic resolutions from typical XAS and XRS data. For the K-edge XAS of Ag, we find nearly complete removal of ∼9.3 eV full width at half maximum broadening from the combined effects of the short core-hole lifetime and instrumental resolution. We are also able to remove nearly all instrumental broadening in an XRS measurement of diamond, with the resulting improved spectrum comparing favorably with prior soft x-ray XAS measurements. We present a practical methodology for implementing the RL algorithm in these problems, emphasizing the importance of testing for stability of the deconvolution process against noise amplification, perturbations in the initial spectra, and uncertainties in the core-hole lifetime

The Galactic Tango: The Elegant Dance of Galaxies and their Supermassive Black Holes

Science.gov (United States)

Sherman, Sydney; Li, Yuexing; Zhu, Qirong

2015-01-01

For well over a decade, it has been known that a supermassive black hole resides in the center of almost every galaxy, and that these black holes strongly correlate with the stellar velocity dispersion (the MBH-σ correlation) and stellar mass (the MBH-Mhost correlation) of their hosts. The origins of these correlations, however, have yet to be determined. To explore the interplay between black holes and galaxies, we have utilized a sample of nearby spiral and elliptical galaxies as well as a sample of AGN in the redshift range z = 0-3. By examining galaxy properties such as mass, kinematics, and growth history, we have determined that these two correlations have distinct origins: the MBH-σ relation may be the result of virial equilibrium, whereas the MBH-Mhost relation may be the result of self-regulated black hole growth and star formation in galaxies. These results confirm the predictions of our previous theoretical model.

Silicon based ultrafast optical waveform sampling

DEFF Research Database (Denmark)

Ji, Hua; Galili, Michael; Pu, Minhao

2010-01-01

A 300 nmx450 nmx5 mm silicon nanowire is designed and fabricated for a four wave mixing based non-linear optical gate. Based on this silicon nanowire, an ultra-fast optical sampling system is successfully demonstrated using a free-running fiber laser with a carbon nanotube-based mode-locker as th......A 300 nmx450 nmx5 mm silicon nanowire is designed and fabricated for a four wave mixing based non-linear optical gate. Based on this silicon nanowire, an ultra-fast optical sampling system is successfully demonstrated using a free-running fiber laser with a carbon nanotube-based mode......-locker as the sampling source. A clear eye-diagram of a 320 Gbit/s data signal is obtained. The temporal resolution of the sampling system is estimated to 360 fs....

Black holes from large N singlet models

Science.gov (United States)

Amado, Irene; Sundborg, Bo; Thorlacius, Larus; Wintergerst, Nico

2018-03-01

The emergent nature of spacetime geometry and black holes can be directly probed in simple holographic duals of higher spin gravity and tensionless string theory. To this end, we study time dependent thermal correlation functions of gauge invariant observables in suitably chosen free large N gauge theories. At low temperature and on short time scales the correlation functions encode propagation through an approximate AdS spacetime while interesting departures emerge at high temperature and on longer time scales. This includes the existence of evanescent modes and the exponential decay of time dependent boundary correlations, both of which are well known indicators of bulk black holes in AdS/CFT. In addition, a new time scale emerges after which the correlation functions return to a bulk thermal AdS form up to an overall temperature dependent normalization. A corresponding length scale was seen in equal time correlation functions in the same models in our earlier work.

Core sample descriptions and summary logs of six wells within the Hanford Reservation

International Nuclear Information System (INIS)

Summers, W.K.; Hanson, R.T.

1977-01-01

From February through May, 1976, selected sites on the Hanford Reservation were core drilled. These six holes provide a loose network of observation holes traversing the reservation in an east--west direction between the Columbia River and State Highway 240. This program represents the first attempt to recover cores from the glaciofluviatile material and Ringold Formation beneath the Hanford Reservation. This contains three parts: an introductory text describing the method of inspection and format for written description; summary logs that illustrate in condensed form the rocks penetrated by the wells drilled; and the detailed written descriptions of core samples. 3 figures, 7 tables

Ultra-fast framing camera tube

Science.gov (United States)

Kalibjian, Ralph

1981-01-01

An electronic framing camera tube features focal plane image dissection and synchronized restoration of the dissected electron line images to form two-dimensional framed images. Ultra-fast framing is performed by first streaking a two-dimensional electron image across a narrow slit, thereby dissecting the two-dimensional electron image into sequential electron line images. The dissected electron line images are then restored into a framed image by a restorer deflector operated synchronously with the dissector deflector. The number of framed images on the tube's viewing screen is equal to the number of dissecting slits in the tube. The distinguishing features of this ultra-fast framing camera tube are the focal plane dissecting slits, and the synchronously-operated restorer deflector which restores the dissected electron line images into a two-dimensional framed image. The framing camera tube can produce image frames having high spatial resolution of optical events in the sub-100 picosecond range.

Concept and methodology for evaluating core damage frequency considering failure correlation at multi units and sites and its application

Energy Technology Data Exchange (ETDEWEB)

Ebisawa, K.; Teragaki, T.; Nomura, S. [Former Incorporated Administrative Agency, Japan Nuclear Safety Organization (Japan); Abe, H., E-mail: Hiroshi_abe@nsr.go.jp [Former Incorporated Administrative Agency, Japan Nuclear Safety Organization (Japan); Shigemori, M.; Shimomoto, M. [Mizuho Information & Research Institute, 2-3, Kanda-Nishikicho, Chiyoda-ku, Tokyo (Japan)

2015-07-15

Highlights: • We develop a method to evaluate CDF considering failure correlation at multi units. • We develop a procedure to evaluate correlation coefficient between multi components. • We evaluate CDF at two different BWR units using correlation coefficients. • We confirm the validity of method and correlation coefficient through the evaluation. - Abstract: The Tohoku earthquake (Mw9.0) occurred on March 11, 2011 and caused a large tsunami. The Fukushima Daiichi Nuclear Power Plant with six units were overwhelmed by the tsunami and core damage occurred. Authors proposed the concept and method for evaluating core damage frequency (CDF) considering failure correlation at the multi units and sites. Based on the above method, one of authors developed the procedure for evaluating the failure correlation coefficient and response correlation coefficient between the multi components under the strong seismic motion. These method and failure correlation coefficients were applied to two different BWR units and their CDF was evaluated by seismic probabilistic risk assessment technology. Through this quantitative evaluation, the validity of the method and failure correlation coefficient was confirmed.

Concept and methodology for evaluating core damage frequency considering failure correlation at multi units and sites and its application

International Nuclear Information System (INIS)

Ebisawa, K.; Teragaki, T.; Nomura, S.; Abe, H.; Shigemori, M.; Shimomoto, M.

2015-01-01

Highlights: • We develop a method to evaluate CDF considering failure correlation at multi units. • We develop a procedure to evaluate correlation coefficient between multi components. • We evaluate CDF at two different BWR units using correlation coefficients. • We confirm the validity of method and correlation coefficient through the evaluation. - Abstract: The Tohoku earthquake (Mw9.0) occurred on March 11, 2011 and caused a large tsunami. The Fukushima Daiichi Nuclear Power Plant with six units were overwhelmed by the tsunami and core damage occurred. Authors proposed the concept and method for evaluating core damage frequency (CDF) considering failure correlation at the multi units and sites. Based on the above method, one of authors developed the procedure for evaluating the failure correlation coefficient and response correlation coefficient between the multi components under the strong seismic motion. These method and failure correlation coefficients were applied to two different BWR units and their CDF was evaluated by seismic probabilistic risk assessment technology. Through this quantitative evaluation, the validity of the method and failure correlation coefficient was confirmed

Magnetic properties of cores from the Wenchuan Earthquake Fault Scientific Drilling Hole-2 (WFSD-2), China

Science.gov (United States)

Zhang, L., Jr.; Sun, Z.; Li, H.; Cao, Y.; Ye, X.; Wang, L.; Zhao, Y.; Han, S.

2015-12-01

During an earthquake, seismic slip and frictional heating may cause the physical and chemical alterations of magnetic minerals within the fault zone. Rock magnetism provides a method for understanding earthquake dynamics. The Wenchuan earthquake Fault Scientific Drilling Project (WFSD) started right after 2008 Mw7.9 Wenchuan earthquake, to investigate the earthquake faulting mechanism. Hole 2 (WFSD-2) is located in the Pengguan Complex in the Bajiaomiao village (Dujiangyan, Sichuan), and reached the Yingxiu-Beichuan fault (YBF). We measured the surface magnetic susceptibility of the cores in WFSD-2 from 500 m to 1530 m with an interval of 1 cm. Rocks at 500-599.31 m-depth and 1211.49-1530 m-depth are from the Neoproterozoic Pengguang Complex while the section from 599.31 m to 1211.49 m is composed of Late Triassic sediments. The magnetic susceptibility values of the first part of the Pengguan Complex range from 1 to 25 × 10-6 SI, while the second part ranges from 10 to 200 × 10-6 SI, which indicate that the two parts are not from the same rock units. The Late Triassic sedimentary rocks have a low magnetic susceptibility values, ranging from -5 to 20 × 10-6 SI. Most fault zones coincide with the high value of magnetic susceptibility in the WFSD-2 cores. Fault rocks, mainly fault breccia, cataclasite, gouge and pseudotachylite within the WFSD-2 cores, and mostly display a significantly higher magnetic susceptibility than host rocks (5:1 to 20:1). In particular, in the YBF zone of the WFSD-2 cores (from 600 to 960 m), dozens of stages with high values of magnetic susceptibility have been observed. The multi-layered fault rocks with high magnetic susceptibility values might indicate that the YBF is a long-term active fault. The magnetic susceptibility values change with different types of fault rocks. The gouge and pseudotachylite have higher values of magnetic susceptibility than other fault rocks. Other primary rock magnetism analyses were then performed to

Drilling and the associated drillhole measurements of the pilot hole ONK-PH6

International Nuclear Information System (INIS)

Oehberg, A.; Hirvonen, H.; Kemppainen, K.; Niemonen, J.; Nordbaeck, N.; Poellaenen, J.; Rouhiainen, P.; Rautio, T.; Tarvainen, A.-M.

2007-08-01

The construction of the ONKALO access tunnel started in September 2004 at Olkiluoto. Most of the investigations related to the construction of the access tunnel aim to ensure successful excavations, reinforcement and sealing. Pilot holes are drillholes, which are core drilled along the tunnel profile. The length of the pilot holes typically varies from several tens of metres to a couple of hundred metres. The pilot holes are aimed to confirm the quality of the rock mass for tunnel construction, and in particular to identify water conductive fractured zones and to provide information that could result in modifications of the existing construction plans. The pilot hole ONK-PH6 was drilled from chainage 1404 to chainage 1559 in September 2006. The length of the hole is 155.04 m. The aim during the drilling work was to orient core samples as much as possible. The deviation of the drillhole was measured during and after the drilling phase. One steering operation by wedging was made at the hole depth of 94.05 metres (top of the wedge). Electric conductivity was measured from the collected returning water samples. Logging of the core samples included the following parameters: lithology, foliation, fracturing, fracture frequency, RQD, fractured zones, core loss and weathering. The rock mechanical logging was based on Q-classification. The tests to determine rock strength and deformation properties were made with a Rock Tester-equipment. Difference Flow method was used for the determination of hydraulic conductivity in fractures and fractured zones in the drillhole. The overlapping i.e. the detailed flow logging mode was used. Besides flow logging Single Point Resistance (SPR), Electric Conductivity (EC) and temperature of the drillhole water were also measured. The flow logging was performed with 0.5 m section length and with 0.1 m depth increment. Water loss tests were conducted in the hole excluding the section 89.04 - 101.04 metres due to the wedge. Geophysical logging

Better late than never: information retrieval from black holes.

Science.gov (United States)

Braunstein, Samuel L; Pirandola, Stefano; Życzkowski, Karol

2013-03-08

We show that, in order to preserve the equivalence principle until late times in unitarily evaporating black holes, the thermodynamic entropy of a black hole must be primarily entropy of entanglement across the event horizon. For such black holes, we show that the information entering a black hole becomes encoded in correlations within a tripartite quantum state, the quantum analogue of a one-time pad, and is only decoded into the outgoing radiation very late in the evaporation. This behavior generically describes the unitary evaporation of highly entangled black holes and requires no specially designed evolution. Our work suggests the existence of a matter-field sum rule for any fundamental theory.

CFD Analysis on a Core Outlet Flow through the Fuel Alignment Plant of SMART

International Nuclear Information System (INIS)

Kim, Y. I.; Bae, Y. M.; Kim, K. K.

2014-01-01

CFD (Computational Fluid Dynamics) simulations were performed to confirm the core flow distribution for SMART, which acquired standard design approval in 2012. In this paper, CFD simulation is also used to calculate the pressure distribution of a core outlet, a Fuel Alignment Plate (FAP), for SMART. In SMART, the fluid discharged from the Steam Generator comes into a Flow Mixing Header Assembly (FMHA), and is rearranged and split into a very fine size. The FMHA is greatly important for enhancing the flow distribution of a downcomer during a normal operation, transient, and even accidents. Then, the fluid discharged from the FMHA flows into the core upstream through flow skirt holes. The Low Core Support Plate (LCSP) reallocates the flow introducing into the inlet core from the core upstream. The deviation of flow distribution becomes smaller or almost disappears by LCSP holes having relatively large loss coefficient compared to the downstream flow deviation. In an open core, the flow deviation at the core inlet region is diminished by cross flow as it goes upward. Near the core outlet, the flow distribution can be distorted by the influence of a Fuel Alignment Plate (FAP) installed above the fuels. In this paper, the effect of the core outlet flow structure such as the FAP holes of SMART is investigated. Before the calculation, the influences of mesh size and turbulence models are inspected. CFD simulations were performed to investigate the effect of FAP flow holes on the core outlet flow of SMART. As a preliminary study, the dependency of the mesh size and turbulence models was tested; a fine grid was applied, the effect of which is negligible, and the core outlet flow is not sensitive to the turbulence models. In brief, the flow resistance of FAP is less than 15% of that of the fuel assemblies. The flow resistance deviation between two flow path patterns is less than 1% of that of active core. Even two flow path patterns located at the downstream location of the

Real-time control of ultrafast laser micromachining by laser-induced breakdown spectroscopy

International Nuclear Information System (INIS)

Tong Tao; Li Jinggao; Longtin, Jon P.

2004-01-01

Ultrafast laser micromachining provides many advantages for precision micromachining. One challenging problem, however, particularly for multilayer and heterogeneous materials, is how to prevent a given material from being ablated, as ultrafast laser micromachining is generally material insensitive. We present a real-time feedback control system for an ultrafast laser micromachining system based on laser-induced breakdown spectroscopy (LIBS). The characteristics of ultrafast LIBS are reviewed and discussed so as to demonstrate the feasibility of the technique. Comparison methods to identify the material emission patterns are developed, and several of the resulting algorithms were implemented into a real-time computer control system. LIBS-controlled micromachining is demonstrated for the fabrication of microheater structures on thermal sprayed materials. Compared with a strictly passive machining process without any such feedback control, the LIBS-based system provides several advantages including less damage to the substrate layer, reduced machining time, and more-uniform machining features

Gauge-Gravity Duality and the Black Hole Interior

Science.gov (United States)

Marolf, Donald; Polchinski, Joseph

2013-10-01

We present a further argument that typical black holes with field theory duals have firewalls at the horizon. This argument makes no reference to entanglement between the black hole and any distant system, and so is not evaded by identifying degrees of freedom inside the black hole with those outside. We also address the Einstein-Rosen=Einstein-Podolsky-Rosen conjecture of Maldacena and Susskind, arguing that the correlations in generic highly entangled states cannot be geometrized as a smooth wormhole.

Spin-controlled ultrafast vertical-cavity surface-emitting lasers

Science.gov (United States)

Höpfner, Henning; Lindemann, Markus; Gerhardt, Nils C.; Hofmann, Martin R.

2014-05-01

Spin-controlled semiconductor lasers are highly attractive spintronic devices providing characteristics superior to their conventional purely charge-based counterparts. In particular, spin-controlled vertical-cavity surface emitting lasers (spin-VCSELs) promise to offer lower thresholds, enhanced emission intensity, spin amplification, full polarization control, chirp control and ultrafast dynamics. Most important, the ability to control and modulate the polarization state of the laser emission with extraordinarily high frequencies is very attractive for many applications like broadband optical communication and ultrafast optical switches. We present a novel concept for ultrafast spin-VCSELs which has the potential to overcome the conventional speed limitation for directly modulated lasers by the relaxation oscillation frequency and to reach modulation frequencies significantly above 100 GHz. The concept is based on the coupled spin-photon dynamics in birefringent micro-cavity lasers. By injecting spin-polarized carriers in the VCSEL, oscillations of the coupled spin-photon system can by induced which lead to oscillations of the polarization state of the laser emission. These oscillations are decoupled from conventional relaxation oscillations of the carrier-photon system and can be much faster than these. Utilizing these polarization oscillations is thus a very promising approach to develop ultrafast spin-VCSELs for high speed optical data communication in the near future. Different aspects of the spin and polarization dynamics, its connection to birefringence and bistability in the cavity, controlled switching of the oscillations, and the limitations of this novel approach will be analysed theoretically and experimentally for spin-polarized VCSELs at room temperature.

Ultrafast Terahertz Conductivity of Photoexcited Nanocrystalline Silicon

DEFF Research Database (Denmark)

Cooke, David; MacDonald, A. Nicole; Hryciw, Aaron

2007-01-01

The ultrafast transient ac conductivity of nanocrystalline silicon films is investigated using time-resolved terahertz spectroscopy. While epitaxial silicon on sapphire exhibits a free carrier Drude response, silicon nanocrystals embedded in glass show a response that is best described by a class...... in the silicon nanocrystal films is dominated by trapping at the Si/SiO2 interface states, occurring on a 1–100 ps time scale depending on particle size and hydrogen passivation......The ultrafast transient ac conductivity of nanocrystalline silicon films is investigated using time-resolved terahertz spectroscopy. While epitaxial silicon on sapphire exhibits a free carrier Drude response, silicon nanocrystals embedded in glass show a response that is best described...

Development of Scanning Ultrafast Electron Microscope Capability.

Energy Technology Data Exchange (ETDEWEB)

Collins, Kimberlee Chiyoko [Sandia National Lab. (SNL-CA), Livermore, CA (United States); Talin, Albert Alec [Sandia National Lab. (SNL-CA), Livermore, CA (United States); Chandler, David W. [Sandia National Lab. (SNL-CA), Livermore, CA (United States); Michael, Joseph R. [Sandia National Lab. (SNL-NM), Albuquerque, NM (United States)

2016-11-01

Modern semiconductor devices rely on the transport of minority charge carriers. Direct examination of minority carrier lifetimes in real devices with nanometer-scale features requires a measurement method with simultaneously high spatial and temporal resolutions. Achieving nanometer spatial resolutions at sub-nanosecond temporal resolution is possible with pump-probe methods that utilize electrons as probes. Recently, a stroboscopic scanning electron microscope was developed at Caltech, and used to study carrier transport across a Si p-n junction [ 1 , 2 , 3 ] . In this report, we detail our development of a prototype scanning ultrafast electron microscope system at Sandia National Laboratories based on the original Caltech design. This effort represents Sandia's first exploration into ultrafast electron microscopy.

White holes and eternal black holes

International Nuclear Information System (INIS)

Hsu, Stephen D H

2012-01-01

We investigate isolated white holes surrounded by vacuum, which correspond to the time reversal of eternal black holes that do not evaporate. We show that isolated white holes produce quasi-thermal Hawking radiation. The time reversal of this radiation, incident on a black hole precursor, constitutes a special preparation that will cause the black hole to become eternal. (paper)

Quantum modeling of ultrafast photoinduced charge separation

Science.gov (United States)

Rozzi, Carlo Andrea; Troiani, Filippo; Tavernelli, Ivano

2018-01-01

Phenomena involving electron transfer are ubiquitous in nature, photosynthesis and enzymes or protein activity being prominent examples. Their deep understanding thus represents a mandatory scientific goal. Moreover, controlling the separation of photogenerated charges is a crucial prerequisite in many applicative contexts, including quantum electronics, photo-electrochemical water splitting, photocatalytic dye degradation, and energy conversion. In particular, photoinduced charge separation is the pivotal step driving the storage of sun light into electrical or chemical energy. If properly mastered, these processes may also allow us to achieve a better command of information storage at the nanoscale, as required for the development of molecular electronics, optical switching, or quantum technologies, amongst others. In this Topical Review we survey recent progress in the understanding of ultrafast charge separation from photoexcited states. We report the state-of-the-art of the observation and theoretical description of charge separation phenomena in the ultrafast regime mainly focusing on molecular- and nano-sized solar energy conversion systems. In particular, we examine different proposed mechanisms driving ultrafast charge dynamics, with particular regard to the role of quantum coherence and electron-nuclear coupling, and link experimental observations to theoretical approaches based either on model Hamiltonians or on first principles simulations.

NEW EQUATIONS OF STATE IN SIMULATIONS OF CORE-COLLAPSE SUPERNOVAE

International Nuclear Information System (INIS)

Hempel, M.; Liebendörfer, M.; Fischer, T.; Schaffner-Bielich, J.

2012-01-01

We discuss three new equations of state (EOS) in core-collapse supernova simulations. The new EOS are based on the nuclear statistical equilibrium model of Hempel and Schaffner-Bielich (HS), which includes excluded volume effects and relativistic mean-field (RMF) interactions. We consider the RMF parameterizations TM1, TMA, and FSUgold. These EOS are implemented into our spherically symmetric core-collapse supernova model, which is based on general relativistic radiation hydrodynamics and three-flavor Boltzmann neutrino transport. The results obtained for the new EOS are compared with the widely used EOS of H. Shen et al. and Lattimer and Swesty. The systematic comparison shows that the model description of inhomogeneous nuclear matter is as important as the parameterization of the nuclear interactions for the supernova dynamics and the neutrino signal. Furthermore, several new aspects of nuclear physics are investigated: the HS EOS contains distributions of nuclei, including nuclear shell effects. The appearance of light nuclei, e.g., deuterium and tritium, is also explored, which can become as abundant as alphas and free protons. In addition, we investigate the black hole formation in failed core-collapse supernovae, which is mainly determined by the high-density EOS. We find that temperature effects lead to a systematically faster collapse for the non-relativistic LS EOS in comparison with the RMF EOS. We deduce a new correlation for the time until black hole formation, which allows the determination of the maximum mass of proto-neutron stars, if the neutrino signal from such a failed supernova would be measured in the future. This would give a constraint for the nuclear EOS at finite entropy, complementary to observations of cold neutron stars.

Development of a Device for a Material Irradiation Test in the OR Test Hole

Energy Technology Data Exchange (ETDEWEB)

Cho, Man Soon; Kang, Y. H.; Kim, B. G.; Choo, K. N.; Sohn, J. M.; Shin, Y. T.; Park, S. J.; Seo, C. K

2008-05-15

To develop a technology and a device for the irradiation test for utilization of the OR/IP holes according to the various requirements of users, the properties of the OR/IP holes were investigated and an irradiation device for the OR hole was designed and fabricated. The OR-4, 5 and the IP-9, 10, 11 holes were selected as those suitable to irradiation tests among the test holes located in the out core area. The conceptual design was performed to design a device to irradiate materials using the OR and IP holes. The capsule for the OR holes is fixed by pressing the protection tube using a clamping device, on the other hand the IP capsule is inserted in the hole without a special clamping device. In the basic design of the irradiation device for the OR hole, the capsules having the outside diameter of 50, 52, 54, 56mm were reviewed theoretically to investigate if they meet the hydraulic and vibration conditions required in the HANARO. The results of the pressure drop test showed that the 3 kinds of capsules having diameter of 52, 54, 56mm satisfied the requirement for the pressure difference and flow rate in HANARO. The capsule of {phi}56mm out of the above three satisfied the vibration condition and was finally selected giving consideration of a capacity of specimens. The capsule having a diameter of {phi}56mm was fabricated and the flow rate was measured. Using the velocity data measured at the out-core facility, the heat transfer coefficient, and the temperature on the surface of the capsule was evaluated to confirm it less than the ONB temperature. As a result, the capsule of {phi}56mm was selected for the irradiation test at the OR holes.

Chirped pulse digital holography for measuring the sequence of ultrafast optical wavefronts

Science.gov (United States)

Karasawa, Naoki

2018-04-01

Optical setups for measuring the sequence of ultrafast optical wavefronts using a chirped pulse as a reference wave in digital holography are proposed and analyzed. In this method, multiple ultrafast object pulses are used to probe the temporal evolution of ultrafast phenomena and they are interfered with a chirped reference wave to record a digital hologram. Wavefronts at different times can be reconstructed separately from the recorded hologram when the reference pulse can be treated as a quasi-monochromatic wave during the pulse width of each object pulse. The feasibility of this method is demonstrated by numerical simulation.

Nonrotating black hole in a post-Newtonian tidal environment

International Nuclear Information System (INIS)

Taylor, Stephanne; Poisson, Eric

2008-01-01

We examine the motion and tidal dynamics of a nonrotating black hole placed within a post-Newtonian external spacetime. The black hole's gravity is described accurately to all orders in Gm/c 2 r, where m is the black-hole mass and r is the distance to the black hole. The tidal perturbation created by the external environment is treated as a small perturbation. At a large distance from the black hole, the gravitational field of the external distribution of matter is assumed to be sufficiently weak to be adequately described by the (first) post-Newtonian approximation to general relativity. There, the black hole is treated as a monopole contribution to the total gravitational field. There exists an overlap in the domains of validity of each description, and the black-hole and post-Newtonian metrics are matched in the overlap. The matching procedure produces (i) a justification of the statement that a nonrotating black hole is a post-Newtonian monopole; (ii) a complete characterization of the coordinate transformation between the inertial, barycentric frame and the accelerated, black-hole frame; (iii) the equations of motion for the black hole; and (iv) the gravito-electric and gravito-magnetic tidal fields acting on the black hole. We first calculate the equations of motion and tidal fields by making no assumptions regarding the nature of the post-Newtonian environment; this could contain a continuous distribution of matter (so as to model a galactic core) or any number of condensed bodies. We next specialize our discussion to a situation in which the black hole is a member of a post-Newtonian two-body system. As an application of our results, we examine the geometry of the deformed event horizon and calculate the tidal heating of the black hole, the rate at which it acquires mass as a result of its tidal interaction with the companion body.

On the theory of hole propagation in an antiferromagnetic background

International Nuclear Information System (INIS)

Kuzemsky, A.L.

1994-10-01

The spectrum of hole quasiparticles and the role of magnetic correlations has been considered in the self-consistent Irreducible Green Functions formalism, motivated from Strongly Correlated Electron systems for correlated electron models of high-Tc superconductivity. The hole quasiparticle dynamics has been discussed for t-J model and compared with that of the spin-fermion model. For this Kondo-Heisenberg-type model it was clearly pointed out on the self-energy level, beyond Hartree-Fock approximation, how the one-and two magnon processes define the true nature of carriers in HTSC. (author). 57 refs

9th International Symposium on Ultrafast Processes in Spectroscopy

CERN Document Server

Silvestri, S; Denardo, G

1996-01-01

This volume is a collection of papers presented at the Ninth International Symposium on "Ultrafast Processes in Spectroscopy" (UPS '95) held at the International Centre for Theo­ retical Physics (ICTP), Trieste (Italy), October 30 -November 3, 1995. These meetings have become recognized as the major forum in Europe for discussion of new work in this rapidly moving field. The UPS'95 Conference in Trieste brought together a multidisciplinary group of researchers sharing common interests in the generation of ultrashort optical pulses and their application to studies of ultrafast phenomena in physics, chemistry, material science, electronics, and biology. It was attended by approximately 250 participants from 20 countries and the five-day program comprises more than 200 papers. The progress of both technology and applications in the field of ultrafast processes during these last years is truly remarkable. The advent of all solid state femtosecond lasers and the extension of laser wavelengths by frequency convers...

Ultrafast Spectroscopic Noninvasive Probe of Vertical Carrier Transport in Heterostructure Devices

Science.gov (United States)

2016-03-01

ARL-TR-7618 ● MAR 2016 US Army Research Laboratory Ultrafast Spectroscopic Noninvasive Probe of Vertical Carrier Transport in...US Army Research Laboratory Ultrafast Spectroscopic Noninvasive Probe of Vertical Carrier Transport in Heterostructure Devices by Blair C...Spectroscopic Noninvasive Probe of Vertical Carrier Transport in Heterostructure Devices 5a. CONTRACT NUMBER 5b. GRANT NUMBER 5c. PROGRAM ELEMENT

Broadband Correlations Provide Evidence for Synchrotron Self-Compton X-rays from the Black Hole Binary GX 339-4

International Nuclear Information System (INIS)

Coriat, M.; Corbel, S.; Buxton, M. M.; Baylin, C. D.

2009-01-01

GX 339-4 has been one of the key sources for unravelling the accretion ejection coupling in accreting stellar mass black holes. After a long period of quiescence between 1999 and 2002, GX 339-4 underwent a series of 4 outbursts that have been intensively observed by many ground based observatories (radio/infrared/optical) and satellites (X-rays). Here, we present some specific results of these broad band observational campaigns, focusing on the optical-infrared/X-ray flux correlations over the four outbursts. Thanks to our extensive data-set, we found a strong OIR/X-ray correlation over four decades with the presence of a break in the correlation index. These results seem to favour a synchrotron self-Compton origin for the X-ray emission in GX 339-4 during the hard state and could also provide an indirect detection of the break frequency in the synchrotron spectrum of the compact jets.

Progress in Ultrafast Intense Laser Science

CERN Document Server

Yamanouchi, Kaoru; Li, Ruxin; Chin, See Leang

2009-01-01

The PUILS series presents Progress in Ultrafast Intense Laser Science, a newly emerging interdisciplinary research field spanning atomic and molecular physics, molecular science, and optical science. PUILS has been stimulated by the recent development of ultrafast laser technologies. Each volume contains approximately 15 chapters, authored by researchers at the forefront. Each chapter opens with an overview of the topics to be discussed, so that researchers, who are not experts in the specific topics, as well as graduate students can grasp the importance and attractions of this sub-field of research, and these are followed by reports of cutting-edge discoveries. This fourth volume covers a broad range of topics from this interdisciplinary research field, focusing on strong field ionization of atoms; excitation, ionization and fragmentation of molecules; nonlinear intense optical phenomena and attosecond pulses; and laser - solid interactions and photoemission.

Localized hole effects in inner-shell excitation

International Nuclear Information System (INIS)

Rescigno, T.N.; Orel, A.E.

1983-01-01

Ab initio calculations of valence shell ionization potentials have shown that orbital relaxation and correlation differences usually make contributions of comparable magnitude. In marked contrast to this observation is the situation for deep core ionization, where correlation differences (approx. 1 eV) play a relatively minor role compared to orbital relaxation (approx. 20 eV). Theoretical calculations have shown that this relaxation is most easily described if the 1s-vacancy created by a K-shell excitation is allowed to localize on one of the atomic centers. For molecules possessing a center of inversion, this means that the molecular orbitals that best describe the final state do not transform as any irreducible representation of the molecular point group. Recent experimental work by Shaw, King, Read and Cvejanovic and by Stefani and coworkers has prompted us to carry out further calculations on N 2 , as well as analogous investigations of 1s/sub N/ → π* excitation in NO and N 2 O. The generalized oscillator strengths display a striking similarity and point to the essential correctness of the localized hole picture for N 2 . The theoretical calculations are briefly described, followed by a summary of the results and comparison to experiment, followed by a short discussion

Phase separation in fermionic systems with particle–hole asymmetry

International Nuclear Information System (INIS)

Montorsi, Arianna

2008-01-01

We determine the ground-state phase diagram of a Hubbard Hamiltonian with correlated hopping, which is asymmetric under particle–hole transform. By lowering the repulsive Coulomb interaction U at appropriate filling and interaction parameters, the ground state separates into hole and electron conducting phases: two different wavevectors characterize the system and charge–charge correlations become incommensurate. By further decreasing U another transition occurs at which the hole conducting region becomes insulating, and conventional phase separation takes place. Finally, for negative U the whole system eventually becomes a paired insulator. It is speculated that such behavior could be at the origin of the incommensurate superconducting phase recently discovered in the 1D Hirsch model. The exact phase boundaries are calculated in one dimension. (letter)

Geologic investigations of drill hole sloughing problems, Nevada Test Site

International Nuclear Information System (INIS)

Drellack, S.L. Jr.; Davies, W.J.; Gonzales, J.L.; Hawkins, W.L.

1983-01-01

Severe sloughing zones encountered while drilling large diameter emplacement holes in Yucca Flat, Nevada Test Site, have been identified, correlated and predicted through detailed geologic investigations. In central and southeastern Area 7 and in northern Area 3, the unstable zones are a very fine-grained, well-sorted, unconsolidated sand deposit, probably eolian in origin, which will readily flow into large diameter drill holes. Other areas exhibit hole erosion related to poor induration or extensive zeolitization of the Tertiary tuff units which are very friable and porous. By examining drill hole samples, geophysical logs, caliper logs and drilling histories, these problem zones can be characterized, correlated and then projected into nearby sites. Maps have been generated to show the depth, thickness and areal extent of these strata. In some cases, they are local and have a lenticular geometry, while in others they are quite extensive. The ability to predict such features can enhance the quality of the hole construction and completion operations to avoid costly delays and the loss of valuable testing real estate. The control of hole enlargements will also eliminate related containment concerns, such as stemming uncertainties

Molten core retention assembly

International Nuclear Information System (INIS)

Lampe, R.F.

1976-01-01

Molten fuel produced in a core overheating accident is caught by a molten core retention assembly consisting of a horizontal baffle plate having a plurality of openings therein, heat exchange tubes having flow holes near the top thereof mounted in the openings, and a cylindrical imperforate baffle attached to the plate and surrounding the tubes. The baffle assembly is supported from the core support plate of the reactor by a plurality of hanger rods which are welded to radial beams passing under the baffle plate and intermittently welded thereto. Preferably the upper end of the cylindrical baffle terminates in an outwardly facing lip to which are welded a plurality of bearings having slots therein adapted to accept the hanger rods

BLACK HOLE MASS ESTIMATES AND RAPID GROWTH OF SUPERMASSIVE BLACK HOLES IN LUMINOUS z ∼ 3.5 QUASARS

Energy Technology Data Exchange (ETDEWEB)

Zuo, Wenwen; Wu, Xue-Bing [Department of Astronomy, School of Physics, Peking University, Beijing 100871 (China); Fan, Xiaohui; Green, Richard [Steward Observatory, The University of Arizona, Tucson, AZ 85721 (United States); Wang, Ran [Kavli Institute for Astronomy and Astrophysics, Peking University, Beijing 100871 (China); Bian, Fuyan [Research School of Astronomy and Astrophysics, Mount Stromlo Observatory, Cotter Road, Weston ACT 2611 (Australia)

2015-02-01

We present new near-infrared (IR) observations of the Hβ λ4861 and Mg II λ2798 lines for 32 luminous quasars with 3.2 < z < 3.9 using the Palomar Hale 200 inch telescope and the Large Binocular Telescope. We find that the Mg II FWHM is well correlated with the Hβ FWHM, confirming itself as a good substitute for the Hβ FWHM in the black hole mass estimates. The continuum luminosity at 5100 Å well correlates with the continuum luminosity at 3000 Å and the broad emission line luminosities (Hβ and Mg II). With simultaneous near-IR spectroscopy of the Hβ and Mg II lines to exclude the influences of flux variability, we are able to evaluate the reliability of estimating black hole masses based on the Mg II line for high redshift quasars. With the reliable Hβ line based black hole mass and Eddington ratio estimates, we find that the z ∼ 3.5 quasars in our sample have black hole masses 1.90 × 10{sup 9} M {sub ☉} ≲ M {sub BH} ≲ 1.37 × 10{sup 10} M {sub ☉}, with a median of ∼5.14 × 10{sup 9} M {sub ☉} and are accreting at Eddington ratios between 0.30 and 3.05, with a median of ∼1.12. Assuming a duty cycle of 1 and a seed black hole mass of 10{sup 4} M {sub ☉}, we show that the z ∼ 3.5 quasars in this sample can grow to their estimated black hole masses within the age of the universe at their redshifts.

Pump polarization insensitive and efficient laser-diode pumped Yb:KYW ultrafast oscillator.

Science.gov (United States)

Wang, Sha; Wang, Yan-Biao; Feng, Guo-Ying; Zhou, Shou-Huan

2016-02-01

We theoretically and experimentally report and evaluate a novel split laser-diode (LD) double-end pumped Yb:KYW ultrafast oscillator aimed at improving the performance of an ultrafast laser. Compared to a conventional unpolarized single-LD end-pumped ultrafast laser system, we improve the laser performance such as absorption efficiency, slope efficiency, cw mode-locking threshold, and output power by this new structure LD-pumped Yb:KYW ultrafast laser. Experiments were carried out with a 1 W output fiber-coupled LD. Experimental results show that the absorption increases from 38.7% to 48.4%, laser slope efficiency increases from 18.3% to 24.2%, cw mode-locking threshold decreases 12.7% from 630 to 550 mW in cw mode-locking threshold, and maximum output-power increases 28.5% from 158.4 to 221.5 mW when we switch the pump scheme from an unpolarized single-end pumping structure to a split LD double-end pumping structure.

REDSHIFT EVOLUTION IN BLACK HOLE-BULGE RELATIONS: TESTING C IV-BASED BLACK HOLE MASSES

International Nuclear Information System (INIS)

Greene, Jenny E.; Peng, Chien Y.; Ludwig, Randi R.

2010-01-01

We re-examine claims for redshift evolution in black hole-bulge scaling relations based on lensed quasars. In particular, we refine the black hole (BH) mass estimates using measurements of Balmer lines from near-infrared spectroscopy obtained with Triplespec at Apache Point Observatory. In support of previous work, we find a large scatter between Balmer and UV line widths, both Mg IIλλ2796, 2803 and C IVλλ1548, 1550. There is tentative evidence that C III]λ1909, despite being a blend of multiple transitions, may correlate well with Mg II, although a larger sample is needed for a real calibration. Most importantly, we find no systematic changes in the estimated BH masses for the lensed sample based on Balmer lines, providing additional support to the interpretation that black holes were overly massive compared to their host galaxies at high redshift.

A CONNECTION BETWEEN PLASMA CONDITIONS NEAR BLACK HOLE EVENT HORIZONS AND OUTFLOW PROPERTIES

Energy Technology Data Exchange (ETDEWEB)

Koljonen, K. I. I.; Russell, D. M.; Bernardini, F. [New York University Abu Dhabi, P.O. Box 129188, Abu Dhabi (United Arab Emirates); Fernández-Ontiveros, J. A. [Istituto di Astrofisica e Planetologia Spaziali (INAF-IAPS), Via Fosso del Cavaliere 100, I-00133 Roma (Italy); Markoff, Sera [Astronomical Institute “Anton Pannekoek”, University of Amsterdam, P.O. Box 94249, 1090 GE Amsterdam (Netherlands); Russell, T. D.; Miller-Jones, J. C. A.; Curran, P. A.; Soria, R. [International Centre for Radio Astronomy Research—Curtin University, GPO Box U1987, Perth, WA 6845 (Australia); Van der Horst, A. J. [Department of Physics, The George Washington University, 725 21st Street NW, Washington, DC 20052 (United States); Casella, P. [INAF, Osservatorio Astronomico di Roma, Via Frascati 33, I-00040 Monteporzio Catone (Italy); Gandhi, P., E-mail: karri.koljonen@nyu.edu [School of Physics and Astronomy, University of Southampton, Highfield, Southampton SO17 1BJ (United Kingdom)

2015-12-01

Accreting black holes are responsible for producing the fastest, most powerful outflows of matter in the universe. The formation process of powerful jets close to black holes is poorly understood, and the conditions leading to jet formation are currently hotly debated. In this paper, we report an unambiguous empirical correlation between the properties of the plasma close to the black hole and the particle acceleration properties within jets launched from the central regions of accreting stellar-mass and supermassive black holes. In these sources the emission of the plasma near the black hole is characterized by a power law at X-ray energies during times when the jets are produced. We find that the photon index of this power law, which gives information on the underlying particle distribution, correlates with the characteristic break frequency in the jet spectrum, which is dependent on magnetohydrodynamical processes in the outflow. The observed range in break frequencies varies by five orders of magnitude in sources that span nine orders of magnitude in black hole mass, revealing a similarity of jet properties over a large range of black hole masses powering these jets. This correlation demonstrates that the internal properties of the jet rely most critically on the conditions of the plasma close to the black hole, rather than other parameters such as the black hole mass or spin, and will provide a benchmark that should be reproduced by the jet formation models.

Multiplane wave imaging increases signal-to-noise ratio in ultrafast ultrasound imaging

International Nuclear Information System (INIS)

Tiran, Elodie; Deffieux, Thomas; Correia, Mafalda; Maresca, David; Osmanski, Bruno-Felix; Pernot, Mathieu; Tanter, Mickael; Sieu, Lim-Anna; Bergel, Antoine; Cohen, Ivan

2015-01-01

Ultrafast imaging using plane or diverging waves has recently enabled new ultrasound imaging modes with improved sensitivity and very high frame rates. Some of these new imaging modalities include shear wave elastography, ultrafast Doppler, ultrafast contrast-enhanced imaging and functional ultrasound imaging. Even though ultrafast imaging already encounters clinical success, increasing even more its penetration depth and signal-to-noise ratio for dedicated applications would be valuable.Ultrafast imaging relies on the coherent compounding of backscattered echoes resulting from successive tilted plane waves emissions; this produces high-resolution ultrasound images with a trade-off between final frame rate, contrast and resolution. In this work, we introduce multiplane wave imaging, a new method that strongly improves ultrafast images signal-to-noise ratio by virtually increasing the emission signal amplitude without compromising the frame rate. This method relies on the successive transmissions of multiple plane waves with differently coded amplitudes and emission angles in a single transmit event. Data from each single plane wave of increased amplitude can then be obtained, by recombining the received data of successive events with the proper coefficients.The benefits of multiplane wave for B-mode, shear wave elastography and ultrafast Doppler imaging are experimentally demonstrated. Multiplane wave with 4 plane waves emissions yields a 5.8  ±  0.5 dB increase in signal-to-noise ratio and approximately 10 mm in penetration in a calibrated ultrasound phantom (0.7 d MHz −1 cm −1 ). In shear wave elastography, the same multiplane wave configuration yields a 2.07  ±  0.05 fold reduction of the particle velocity standard deviation and a two-fold reduction of the shear wave velocity maps standard deviation. In functional ultrasound imaging, the mapping of cerebral blood volume results in a 3 to 6 dB increase of the contrast-to-noise ratio in

Tracking ultrafast relaxation dynamics of furan by femtosecond photoelectron imaging

International Nuclear Information System (INIS)

Liu, Yuzhu; Knopp, Gregor; Qin, Chaochao; Gerber, Thomas

2015-01-01

Graphical abstract: - Highlights: • Relaxation dynamics of furan are tracked by femtosecond photoelectron imaging. • The mechanism for ultrafast formation of α-carbene and β-carbene is proposed. • Ultrafast internal conversion from S 2 to S 1 is observed. • The transient characteristics of the fragment ions are obtained. • Single-color multi-photon ionization dynamics at 800 nm are also studied. - Abstract: Ultrafast internal conversion dynamics of furan has been studied by femtosecond photoelectron imaging (PEI) coupled with photofragmentation (PF) spectroscopy. Photoelectron imaging of single-color multi-photon ionization and two-color pump–probe ionization are obtained and analyzed. Photoelectron bands are assigned to the related states. The time evolution of the photoelectron signal by pump–probe ionization can be well described by a biexponential decay: two rapid relaxation pathways with time constants of ∼15 fs and 85 (±11) fs. The rapid relaxation is ascribed to the ultrafast internal conversion (IC) from the S 2 state to the vibrationally hot S 1 state. The second relaxation process is attributed to the redistributions and depopulation of secondarily populated high vibronic S 1 state and the formation of α-carbene and β-carbene by H immigration. Additionally, the transient characteristics of the fragment ions are also measured and discussed as a complementary understanding

Fast MR imaging and ultrafast MR imaging of fetal central nervous system abnormalities

Energy Technology Data Exchange (ETDEWEB)

Shakudo, Miyuki; Manabe, Takao; Murata, Katsuko; Matsuo, Ryoichi; Oda, Junro [Osaka City General Hospital (Japan); Inoue, Yuichi; Mochizuki, Kunizo; Yamada, Ryusaku

2001-12-01

The aims of this study were two: to compare the efficacy of fast MRI (breath-hold fast spin-echo T2-weighted and fast gradient-echo T1-weighted sequence) and ultrafast MRI (half-Fourier acquisition single-shot turbo spin-echo sequence) in evaluation of fetal central nervous system (CNS) abnormalities at late gestational age, and to compare the capability of fast MRI and ultrafast MRI to assess fetal CNS abnormalities with that of prenatal ultrasonography (US). Forty-nine women with fetuses at gestational ages of 26-39 weeks underwent fast MRI (29 patients) or ultrafast MRI (20 patients). In detection of motion artifact, visualization of the lateral and 4th ventricles, and differentiation between gray and white matter in cerebral hemispheres, ultrafast MRI was significantly superior to fast MRI (p<0.0001, Mann-Whitney U test). In 25 of 43 cases, US and MR diagnoses were the same and consistent with postnatal diagnosis. In 10 of 43 cases, MRI demonstrated findings additional to or different from those of US, and MR findings were confirmed postnatally. MRI, particularly ultrafast MRI, is useful for demonstrating CNS abnormalities in situations in which US is suggestive but not definitive. (author)

State-Resolved Metal Nanoparticle Dynamics Viewed through the Combined Lenses of Ultrafast and Magneto-optical Spectroscopies.

Science.gov (United States)

Zhao, Tian; Herbert, Patrick J; Zheng, Hongjun; Knappenberger, Kenneth L

2018-05-08

Electronic carrier dynamics play pivotal roles in the functional properties of nanomaterials. For colloidal metals, the mechanisms and influences of these dynamics are structure dependent. The coherent carrier dynamics of collective plasmon modes for nanoparticles (approximately 2 nm and larger) determine optical amplification factors that are important to applied spectroscopy techniques. In the nanocluster domain (sub-2 nm), carrier coupling to vibrational modes affects photoluminescence yields. The performance of photocatalytic materials featuring both nanoparticles and nanoclusters also depends on the relaxation dynamics of nonequilibrium charge carriers. The challenges for developing comprehensive descriptions of carrier dynamics spanning both domains are multifold. Plasmon coherences are short-lived, persisting for only tens of femtoseconds. Nanoclusters exhibit discrete carrier dynamics that can persist for microseconds in some cases. On this time scale, many state-dependent processes, including vibrational relaxation, charge transfer, and spin conversion, affect carrier dynamics in ways that are nonscalable but, rather, structure specific. Hence, state-resolved spectroscopy methods are needed for understanding carrier dynamics in the nanocluster domain. Based on these considerations, a detailed understanding of structure-dependent carrier dynamics across length scales requires an appropriate combination of spectroscopic methods. Plasmon mode-specific dynamics can be obtained through ultrafast correlated light and electron microscopy (UCLEM), which pairs interferometric nonlinear optical (INLO) with electron imaging methods. INLO yields nanostructure spectral resonance responses, which capture the system's homogeneous line width and coherence dynamics. State-resolved nanocluster dynamics can be obtained by pairing ultrafast with magnetic-optical spectroscopy methods. In particular, variable-temperature variable-field (VTVH) spectroscopies allow quantification

Two stellar-mass black holes in the globular cluster M22.

Science.gov (United States)

Strader, Jay; Chomiuk, Laura; Maccarone, Thomas J; Miller-Jones, James C A; Seth, Anil C

2012-10-04

Hundreds of stellar-mass black holes probably form in a typical globular star cluster, with all but one predicted to be ejected through dynamical interactions. Some observational support for this idea is provided by the lack of X-ray-emitting binary stars comprising one black hole and one other star ('black-hole/X-ray binaries') in Milky Way globular clusters, even though many neutron-star/X-ray binaries are known. Although a few black holes have been seen in globular clusters around other galaxies, the masses of these cannot be determined, and some may be intermediate-mass black holes that form through exotic mechanisms. Here we report the presence of two flat-spectrum radio sources in the Milky Way globular cluster M22, and we argue that these objects are black holes of stellar mass (each ∼10-20 times more massive than the Sun) that are accreting matter. We find a high ratio of radio-to-X-ray flux for these black holes, consistent with the larger predicted masses of black holes in globular clusters compared to those outside. The identification of two black holes in one cluster shows that ejection of black holes is not as efficient as predicted by most models, and we argue that M22 may contain a total population of ∼5-100 black holes. The large core radius of M22 could arise from heating produced by the black holes.

Ultrafast biophotonics

CERN Document Server

Vasa, P

2016-01-01

This book presents emerging contemporary optical techniques of ultrafast science which have opened entirely new vistas for probing biological entities and processes. The spectrum reaches from time-resolved imaging and multiphoton microscopy to cancer therapy and studies of DNA damage. The book displays interdisciplinary research at the interface of physics and biology. Emerging topics on the horizon are also discussed, like the use of squeezed light, frequency combs and terahertz imaging as the possibility of mimicking biological systems. The book is written in a manner to make it readily accessible to researchers, postgraduate biologists, chemists, engineers, and physicists and students of optics, biomedical optics, photonics and biotechnology.

Ultra-fast ipsilateral DPOAE adaptation not modulated by attention?

Science.gov (United States)

Dalhoff, Ernst; Zelle, Dennis; Gummer, Anthony W.

2018-05-01

Efferent stimulation of outer hair cells is supposed to attenuate cochlear amplification of sound waves and is accompanied by reduced DPOAE amplitudes. Recently, a method using two subsequent f2 pulses during presentation of a longer f1 pulse was introduced to measure fast ipsilateral adaptation effects on separated DPOAE components. Compensating primary-tone onsets for their latencies at the f2-tonotopic place, the average adaptation measured in four normal-hearing subjects was 5.0 dB with a time constant below 5 ms. In the present study, two experiments were performed to determine the origin of this ultra-fast ipsilateral adaptation effect. The first experiment measured ultra-fast ipsilateral adaptation using a two-pulse paradigm at three frequencies in the four subjects, while controlling for visual attention of the subjects. The other experiment also controlled for visual attention, but utilized a sequence of f2 short pulses in the presence of a continuous f1 tone to sample ipsilateral adaptation effects with longer time constants in eight subjects. In the first experiment, no significant change in the ultra-fast adaptation between non-directed attention and visual attention could be detected. In contrast, the second experiment revealed significant changes in the magnitude of the slower ipsilateral adaptation in the visual-attention condition. In conclusion, the lack of an attentional influence indicates that the ultra-fast ipsilateral DPOAE adaptation is not solely mediated by the medial olivocochlear reflex.

Assessment of Two-Phase Flow Heat Transfer Correlations for Molten Core-Concrete Interaction Study

International Nuclear Information System (INIS)

Tourniaire, B.; Varo, O.

2006-01-01

The prediction of heat transfer between corium pool and concrete basemat is of particular significance in the framework of the study of PWR's severe accident. Heat transfer directly governs the ablation velocity of concrete in case of molten core-concrete interaction (MCCI) and, consequently, the time delay when the reactor cavity may fail. From a restricted hydrodynamic point of view, this issue is related to heat transfer between a heated bubbling pool and a porous wall with gas injection. Several experimental studies have been performed with simulant materials and many correlations have been provided to address this issue. The main purpose of this paper is to assess these correlations from comparisons against the available experimental data. After a review of these data, the different correlations are presented. Attention focuses here on the correlations generally used in MCCI study: Kutateladze-Malenkov, Konsetov and BALI correlations. The Deckwer's correlation is also included in this review. The comparisons between the results of these correlations and the experimental data are then discussed. (authors)

Black Hole Horizons and Bose-Einstein Condensation

CERN Document Server

Ferrari, Frank

2016-01-01

Consider a particle sitting at a fixed position outside of a stable black hole. If the system is heated up, the black hole horizon grows and there should exist a critical temperature above which the particle enters the black hole interior. We solve a simple model describing exactly this situation: a large N matrix quantum mechanics modeling a fixed D-particle in a black hole background. We show that indeed a striking phenomenon occurs: above some critical temperature, there is a non-perturbative Bose-Einstein condensation of massless strings. The transition, even though precisely defined by the presence of the condensate, cannot be sharply detected by measurements made in a finite amount of time. The order parameter is fundamentally non-local in time and corresponds to infinite-time correlations.

Analysis of the equalizing holes resistance in fuel assembly spike for lead-based reactor

International Nuclear Information System (INIS)

Zhang, Guangyu; Jin, Ming; Wang, Jianye; Song, Yong

2017-01-01

Highlights: • A RELAP5 model for a 10 MWth lead-based reactor was built to study the hydrodynamic characteristics between the equalizing holes in the fuel assembly spike. • Different fuel assembly total blockage scenarios and different resistances for different fuel assemblies were examined. • The inherent safety characteristics of the lead-based reactor was improved by optimizing the configuration of equalizing holes in the fuel assembly spike. - Abstract: To avoid the damage of the fuel rod cladding when a fuel assembly (FA) is totally blocked, a special configuration of the fuel assembly spike was designed with some equalizing holes in the center region which can let the coolant to flow during the totally blockage scenarios of FA. To study the hydrodynamic characteristics between the equalizing holes and an appropriate resistance, a RELAP5 model was developed for a 10 MWth lead-based reactor which used lead-bismuth as coolant. Several FA total blockage and partial core blockage scenarios were selected. The simulation results indicated that when all the FA spike equalizing holes had the same hydraulic resistance, only a narrow range of suitable equalizing holes resistances could be chosen when a FA was blocked. However, in the two or more FA blockage scenarios, there were no appropriate resistances to meet the requirement. In addition, with different FA spike equalizing holes with different resistances, a large range of suitable equalizing hole resistances could be chosen. Especially a series of suitable resistances were selected when the small power FA resistance was 1/2, 1/4, 1/8 of the large one. Under these circumstances, one, two or three FA blockages would not damage the core. These demonstrated that selecting a series of suitable hydraulic resistances for the equalizing holes could improve the safety characteristics of the reactor effectively.

Borehole-calibration methods used in cased and uncased test holes to determine moisture profiles in the unsaturated zone, Yucca Mountain, Nevada

International Nuclear Information System (INIS)

Hammermeister, D.P.; Kneiblher, C.R.; Klenke, J.

1985-01-01

The use of drilling and coring methods that minimize the disturbance of formation rock and core has permitted field calibration of neutron-moisture tools in relatively large diameter cased and uncased boreholes at Yucca Mountain, Nevada. For 5.5-inch diameter cased holes, there was reasonable agreement between a field calibration in alluvium-colluvium and a laboratory calibration in a chamber containing silica sand. There was little difference between moisture-content profiles obtained in a neutron-access hole with a hand-held neutron-moisture meter and an automated borehole-logging tool using laboratory-generated calibration curves. Field calibrations utilizing linear regression analyses and as many as 119 data pairs show a good correlation between neutron-moisture counts and volumetric water content for sections of uncased 6-inch diameter boreholes in nonwelded and bedded tuff. Regression coefficients ranged from 0.80 to 0.94. There were only small differences between calibration curves in 4.25- and 6-inch uncased sections of boreholes. Results of analyzing field calibration data to determine the effects of formation density on calibration curves were inconclusive. Further experimental and theoretical work is outlined

Mineralogy of drill hole UE-25pnumber1 at Yucca Mountain, Nevada

International Nuclear Information System (INIS)

Chipera, S.J.; Bish, D.L.

1988-05-01

Drill hole UE-25p/number sign/1 is located east of the candidate repository block at Yucca Mountain, Nevada, and as such provides information on the geology of the accessible environment. The hole was drilled to a depth of 1807 m (5923 ft) and is unique in that it penetrates tuffs that are older than any volcanic units previously encountered in drill holes at Yucca Mountain. In addition, it is the only hole drilled to date that penetrates the base of the tuff sequence and enters the underlying Paleozoic dolomite basement. We have examined the mineralogy of drill cuttings, core, and sidewall samples from drill hole UE-25p/number sign/1 is similar to that in the other drill holes examined at Yucca Mountain. The only significant differences in mineralogy from other drill holes include the presence of dolomite in the Paleozoic carbonate rocks and the occurrence of up to 3% laumontite, a Ca-zeolite, in four samples of the Lithic Ridge Tuff. 15 refs., 5 figs., 4 tabs

One particle-hole excitations in p- and fp-shell nuclei

International Nuclear Information System (INIS)

Hees, A.G.M. van.

1982-01-01

Results are presented of shell model calculations of medium and light atomic nuclei. The influence of the allowance of one particle-hole excitations is investigated. This enables improved descriptions of intermediate mass nuclei in the fp-shell. For light p-shell nuclei one particle-hole excitations create exclusively situations with abnormal parity. The description of situations with normal parity is not changed by enlarging the model space. In the first chapter shell-model calculations are performed on the light Ni-isotopes (A = 57-59). One nucleon is allowed to be excited from the fsub(7/2) orbit to one of the other fp-shell orbits. The general observation in the enlarged model space is that one can use operators that require a much weaker 'renormalization' and the calculation requires only a selected set of matrix elements of the Hamiltonian. An additional advantage of the inclusion of one particle-hole excitations is that it allows a description of several intruder states, i.e. states that cannot be produced with the assumption of a closed 56 Ni core. In the second chapter the nuclei with mass number A = 52-55, i.e. a small number of holes in the 56 Ni core, are investigated similarly. In the third chapter much lighter nuclei (A = 4-16) are discussed. For a theoretical description of nonnormal-parity states one has to admit the excitation of at least one nucleon to a higher harmonic-oscillator major-shell. (Auth.)

Advanced ultrafast fiber laser sources enabled by fiber nonlinearities

International Nuclear Information System (INIS)

Liu, Wei

2017-05-01

Development of high power/energy ultrafast fiber lasers for scientific research and industrial applications is one of the most exciting fields in ultrafast optics. This thesis demonstrated new means to improve two essential properties - which are indispensable for novel applications such as high-harmonic generation (HHG) and multiphoton microscopy (MPM) - of an ultrafast fiber laser system: energy scaling capability and wavelength tunability. High photon-flux extreme ultraviolet sources enabled by HHG desire high power (>100 W), high repetition-rate (>1 MHz) ultrafast driving laser sources. We have constructed from scratch a high-power Yb-fiber laser system using the well-known chirped-pulse amplification (CPA) technique. Such a CPA system capable of producing ∝200-W average power consists of a monolithic Yb-fiber oscillator, an all-fiber stretcher, a pre-amplifier chain, a main amplifier constructed from rode-type large pitch fiber, and a diffraction-grating based compressor. To increase the HHG efficiency, ultrafast pulses with duration 130-W average power. The amplified pulses are compressed to 60-fs pulses with 100-W average power, constituting a suitable HHG driving source. MPM is a powerful biomedical imaging tool, featuring larger penetration depth while providing the capability of optical sectioning. Although femtosecond solid-state lasers have been widely accepted as the standard option as MPM driving sources, fiber-based sources have received growing research efforts due to their superior performance. In the second part of this thesis, we both theoretically and experimentally demonstrated a new method of producing wavelength widely tunable femtosecond pulses for driving MPM. We employed self-phase modulation to broaden a narrowband spectrum followed by bandpass filters to select the rightmost/leftmost spectral lobes. Widely tunable in 820-1225 nm, the resulting sources generated nearly transform-limited, ∝100 fs pulses. Using short fibers with large

Octave-Spanning Mid-IR Supercontinuum Generation with Ultrafast Cascaded Nonlinearities

DEFF Research Database (Denmark)

Zhou, Binbin; Guo, Hairun; Liu, Xing

2014-01-01

An octave-spanning mid-IR supercontinuum is observed experimentally using ultrafast cascaded nonlinearities in an LiInS2 quadratic nonlinear crystal pumped with 70 fs energetic mid-IR pulses and cut for strongly phase-mismatched second-harmonic generation.......An octave-spanning mid-IR supercontinuum is observed experimentally using ultrafast cascaded nonlinearities in an LiInS2 quadratic nonlinear crystal pumped with 70 fs energetic mid-IR pulses and cut for strongly phase-mismatched second-harmonic generation....

Holographic shell model: Stack data structure inside black holes?

Science.gov (United States)

Davidson, Aharon

2014-03-01

Rather than tiling the black hole horizon by Planck area patches, we suggest that bits of information inhabit, universally and holographically, the entire black core interior, a bit per a light sheet unit interval of order Planck area difference. The number of distinguishable (tagged by a binary code) configurations, counted within the context of a discrete holographic shell model, is given by the Catalan series. The area entropy formula is recovered, including Cardy's universal logarithmic correction, and the equipartition of mass per degree of freedom is proven. The black hole information storage resembles, in the count procedure, the so-called stack data structure.

Quantum chaos and the black hole horizon

CERN Multimedia

CERN. Geneva

2016-01-01

Thanks to AdS/CFT, the analogy between black holes and thermal systems has become a practical tool, shedding light on thermalization, transport, and entanglement dynamics. Continuing in this vein, recent work has shown how chaos in the boundary CFT can be analyzed in terms of high energy scattering right on the horizon of the dual black hole. The analysis revolves around certain out-of-time-order correlation functions, which are simple diagnostics of the butterfly effect. We will review this work, along with a general bound on these functions that implies black holes are the most chaotic systems in quantum mechanics. (NB Room Change to Main Auditorium)

Gamma Ray Bursts and the Birth of Black Holes

Science.gov (United States)

Gehrels, Neil

2009-01-01

Black holes have been predicted since the 1940's from solutions of Einstein's general relativity field equation. There is strong evidence of their existence from astronomical observations, but their origin has remained an open question of great interest. Gamma-ray bursts may the clue. They are powerful explosions, visible to high redshift, and appear to be the birth cries of black holes. The Swift and Fermi missions are two powerful NASA observatories currently in orbit that are discovering how gamma-ray bursts work. Evidence is building that the long and short duration subcategories of GRBs have very different origins: massive star core collapse to a black hole for long bursts and binary neutron star coalescence to a black hole for short bursts. The similarity to Type II and Ia supernovae originating from young and old stellar progenitors is striking. Bursts are tremendously luminous and are providing a new tool to study the high redshift universe. One Swift burst at z=8.3 is the most distant object known in the universe. The talk will present the latest gamma-ray burst results from Swift and Fermi and will highlight what they are teaching us about black holes and jet outflows.

Photonic-assisted ultrafast THz wireless access

DEFF Research Database (Denmark)

Yu, Xianbin; Chen, Ying; Galili, Michael

THz technology has been considered feasible for ultrafast wireless data communi- cation, to meet the increasing demand on next-generation fast wireless access, e.g., huge data file transferring and fast mobile data stream access. This talk reviews recent progress in high-speed THz wireless...

Detailed cross sections of the Eocene Green River Formation along the north and east margins of the Piceance Basin, western Colorado, using measured sections and drill hole information

Science.gov (United States)

Johnson, Ronald C.

2014-01-01

This report presents two detailed cross sections of the Eocene Green River Formation in the Piceance Basin, northwestern Colorado, constructed from eight detailed measured sections, fourteen core holes, and two rotary holes. The Eocene Green River Formation in the Piceance Basin contains the world’s largest known oil shale deposit with more than 1.5 billion barrels of oil in place. It was deposited in Lake Uinta, a long-lived saline lake that once covered much of the Piceance Basin and the Uinta Basin to the west. The cross sections extend across the northern and eastern margins of the Piceance Basin and are intended to aid in correlating between surface sections and the subsurface in the basin.

Study of the ultrafast polarization dynamics in lithium borohydride by means of femtosecond X-ray diffraction

International Nuclear Information System (INIS)

Stingl, Johannes

2013-01-01

In this thesis the ultrafast electronic polarisation in the crystalline material lithium borohydride (LiBH 4 ) is examined. The material is excited by a femtosecond long optical pulse and scanned by a likewise short X-ray pulse. Using X-ray scattering the optically induced spatial rearrangement of electronic charge can be directly mapped with atomic spatial resolution. Copper K-alpha X-rays for the experiment are produced in a laboratory table-top laserplasma source with 1 kHz repetition rate. This radiation is then focused on a powdered sample. Debye-Scherrer rings produced from powder diffraction are collected on a large area detector and processed to yield intensity profiles. Using pump-probe technique the change in diffracted intensity, triggered by excitation with a femtosecond optical pulse is examined. The temporal resolution is given by the delay between pump and probe pulse. This way insight is gained into the dynamic electronic evolution of the system. Intensity changes can be correlated to changes in charge density in the relevant material to elucidate structural dynamics on the femtosecond time scale. Lithium borohydride was chosen since it displays necessary characteristics for the exploration of ultrafast electronic polarisation. Up to date there has been no spatially resolved research in the femtosecond regime elucidating this electronic phenomenon. This work presents the ultrafast resonse in Lithiumborhydrid (LiBH 4 ) to strong electronic fields with optical frequencies, which leads to charge relocation accompanied by electronic polarisation.

Evaluation of chronic pulmonary emphysema ultrafast computed tomography

International Nuclear Information System (INIS)

Tsuchida, Fumihiro; Yagyu, Hisanaga; Ohishi, Shuji; Nakamura, Hiroyuki; Matsuoka, Takeshi

2003-01-01

We compared pulmonary ventilation dynamics between 41 patients with pulmonary emphysema and 11 healthy subjects with normal pulmonary function using ultrafast computed tomography (CT). Regions of interest (ROIs) for multislice scanning were selected from the anatomical levels of the carina in the right upper lung field. Several identical slices were selected from the inspiratory and expiratory scans. The average CT values in the ROIs (AvROI) were obtained during the inspiratory phase (inAvROI) and the expiratory phase (exAvROI. The ratio of change from inAvROI to exAvROI ((I-E)/E ratio) was also used for image analysis. Furthermore, possible correlations between the CT image parameters and pulmonary function test parameters were examined. The results showed that the exAvROI and inAvROI values and (I-E)/E ratio were lower in the emphysema group than in the normal pulmonary function group. Among the image data parameters, the exAvROI value correlated most closely with pulmonary function parameters, in particular, with the pulmonary diffusing capacity. These findings suggest that image data parameters of ventilation dynamics may be useful for evaluating the severity of pulmonary emphysema. (author)

Discrete decoding based ultrafast multidimensional nuclear magnetic resonance spectroscopy

International Nuclear Information System (INIS)

Wei, Zhiliang; Lin, Liangjie; Ye, Qimiao; Li, Jing; Cai, Shuhui; Chen, Zhong

2015-01-01

The three-dimensional (3D) nuclear magnetic resonance (NMR) spectroscopy constitutes an important and powerful tool in analyzing chemical and biological systems. However, the abundant 3D information arrives at the expense of long acquisition times lasting hours or even days. Therefore, there has been a continuous interest in developing techniques to accelerate recordings of 3D NMR spectra, among which the ultrafast spatiotemporal encoding technique supplies impressive acquisition speed by compressing a multidimensional spectrum in a single scan. However, it tends to suffer from tradeoffs among spectral widths in different dimensions, which deteriorates in cases of NMR spectroscopy with more dimensions. In this study, the discrete decoding is proposed to liberate the ultrafast technique from tradeoffs among spectral widths in different dimensions by focusing decoding on signal-bearing sites. For verifying its feasibility and effectiveness, we utilized the method to generate two different types of 3D spectra. The proposed method is also applicable to cases with more than three dimensions, which, based on the experimental results, may widen applications of the ultrafast technique

Discrete decoding based ultrafast multidimensional nuclear magnetic resonance spectroscopy

Science.gov (United States)

Wei, Zhiliang; Lin, Liangjie; Ye, Qimiao; Li, Jing; Cai, Shuhui; Chen, Zhong

2015-07-01

The three-dimensional (3D) nuclear magnetic resonance (NMR) spectroscopy constitutes an important and powerful tool in analyzing chemical and biological systems. However, the abundant 3D information arrives at the expense of long acquisition times lasting hours or even days. Therefore, there has been a continuous interest in developing techniques to accelerate recordings of 3D NMR spectra, among which the ultrafast spatiotemporal encoding technique supplies impressive acquisition speed by compressing a multidimensional spectrum in a single scan. However, it tends to suffer from tradeoffs among spectral widths in different dimensions, which deteriorates in cases of NMR spectroscopy with more dimensions. In this study, the discrete decoding is proposed to liberate the ultrafast technique from tradeoffs among spectral widths in different dimensions by focusing decoding on signal-bearing sites. For verifying its feasibility and effectiveness, we utilized the method to generate two different types of 3D spectra. The proposed method is also applicable to cases with more than three dimensions, which, based on the experimental results, may widen applications of the ultrafast technique.

Ultrafast Mid-IR Nonlinear Optics in Gas-filled Hollow-core Photonic Crystal Fibers

DEFF Research Database (Denmark)

Habib, Selim

Invention of hollow-core fiber has been proven an ideal medium to study light-gas interaction. Tight confinement of light inside hollowcore fiber allows unremitting and tailored interaction between light and gas over long distances. In this work, we used a special kind of hollowcore fiber − hollow......-core anti-resonant (HC-AR) fiber to study the various nonlinear effects filled with Raman free noble gas. One of the main striking features of HC-AR fiber is that ∼99.99% light can be guided inside the central hollow-core region, which significantly enhances damage threshold level. HC-AR fiber can sustain...... be tuned by simply changing the pressure of the gas while at the same time providing extremely wide transparency ranges. In this thesis, we propose several low-loss broadband guidance HC-AR fibers and investigate soliton-plasma dynamics using HC-AR fiber filled with noble gas in the mid-IR. The combined...

Photodissociation dynamics of core-excited molecular oxygen

International Nuclear Information System (INIS)

Coutinho, L.H.; Homem, M.G.P.; Marinho, R.R.T.; Mocellin, A.; Naves de Brito, A.; Burmeister, F.

2004-01-01

Full text: The fragmentation of molecules after the excitation of a core orbital is of particular interest due to the localization of these orbitals and the possibility to observe dissociation in the same time scale as the electronic decay. This process, which occurs in a few femtoseconds and is known as ultrafast dissociation, has been observed for O 2 and the results will be presented. We used the PhotoElectron-PhotoIon COincidence (PEPICO) and PhotoElectron-PhotoIon-PhotoIon COincidence (PEPIPICO) spectroscopy technique to analyze the produced fragments in the 529 to 540 eV photon energy range. Usually Electron Spectroscopy (ES) is employed to establish whether this peculiar phenomenon occurs or not. Here we successfully put forward the use of partial ion yield (PIY) spectroscopy to investigate ultrafast dissociation. The experiment was performed at the Brazilian Synchrotron Light Laboratory (LNLS). The SGM beamline was equipped with an end-station composed by a time-of-flight mass spectrometer able to rotate with respect to the polarization of the exciting beam. The measurements were taken with the TOF axis performing an angle of 54.7 deg with respect to the polarization vector of the light. The data were corrected for non-unitary detection efficiency in the detectors

Tracking ultrafast relaxation dynamics of furan by femtosecond photoelectron imaging

Energy Technology Data Exchange (ETDEWEB)

Liu, Yuzhu, E-mail: yuzhu.liu@gmail.com [School of Physics and Optoelectronic Engineering, Nanjing University of Information Science and Technology, Nanjing 210044 (China); Knopp, Gregor [Paul Scherrer Institute, Villigen 5232 (Switzerland); Qin, Chaochao [Department of Physics, Henan Normal University, Xinxiang 453007 (China); Gerber, Thomas [Paul Scherrer Institute, Villigen 5232 (Switzerland)

2015-01-13

Graphical abstract: - Highlights: • Relaxation dynamics of furan are tracked by femtosecond photoelectron imaging. • The mechanism for ultrafast formation of α-carbene and β-carbene is proposed. • Ultrafast internal conversion from S{sub 2} to S{sub 1} is observed. • The transient characteristics of the fragment ions are obtained. • Single-color multi-photon ionization dynamics at 800 nm are also studied. - Abstract: Ultrafast internal conversion dynamics of furan has been studied by femtosecond photoelectron imaging (PEI) coupled with photofragmentation (PF) spectroscopy. Photoelectron imaging of single-color multi-photon ionization and two-color pump–probe ionization are obtained and analyzed. Photoelectron bands are assigned to the related states. The time evolution of the photoelectron signal by pump–probe ionization can be well described by a biexponential decay: two rapid relaxation pathways with time constants of ∼15 fs and 85 (±11) fs. The rapid relaxation is ascribed to the ultrafast internal conversion (IC) from the S{sub 2} state to the vibrationally hot S{sub 1} state. The second relaxation process is attributed to the redistributions and depopulation of secondarily populated high vibronic S{sub 1} state and the formation of α-carbene and β-carbene by H immigration. Additionally, the transient characteristics of the fragment ions are also measured and discussed as a complementary understanding.

The effect of optical system design for laser micro-hole drilling process

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