Quantum computation with two-dimensional graphene quantum dots
Institute of Scientific and Technical Information of China (English)
Li Jie-Sen; Li Zhi-Bing; Yao Dao-Xin
2012-01-01
We study an array of graphene nano sheets that form a two-dimensional S =1/2 Kagome spin lattice used for quantum computation.The edge states of the graphene nano sheets axe used to form quantum dots to confine electrons and perform the computation.We propose two schemes of bang-bang control to combat decoherence and realize gate operations on this array of quantum dots.It is shown that both schemes contain a great amount of information for quantum computation.The corresponding gate operations are also proposed.
Magnetic quantum dot in two-dimensional topological insulators
Li, Guo; Zhu, Jia-Lin; Yang, Ning
2017-03-01
Magnetic quantum dots in two-dimensional band and topological insulators are studied by solving the modified Dirac model under nonuniform magnetic fields. The Landau levels split into discrete states with certain angular momentum. The states splitting from the zero Landau levels lie in the energy gap for topological insulators but are out of the gap for band insulators. It is found that the ground states oscillate between the spin-up and spin-down states when the magnetic field or the dot size changes. The oscillation manifests itself as changes of sign and strength of charge currents near the dot's edge.
Soliton nanoantennas in two-dimensional arrays of quantum dots
Gligorić, G; Hadžievski, Lj; Slepyan, G Ya; Malomed, B A
2015-01-01
We consider two-dimensional (2D) arrays of self-organized semiconductor quantum dots (QDs) strongly interacting with electromagnetic field in the regime of Rabi oscillations. The QD array built of two-level states is modelled by two coupled systems of discrete nonlinear Schr\\"{o}dinger equations. Localized modes in the form of single-peaked fundamental and vortical stationary Rabi solitons and self-trapped breathers have been found. The results for the stability, mobility and radiative properties of the Rabi modes suggest a concept of a self-assembled 2D \\textit{% soliton-based nano-antenna}, which should be stable against imperfections In particular, we discuss the implementation of such a nano-antenna in the form of surface plasmon solitons in graphene, and illustrate possibilities to control their operation by means of optical tools.
Optical Two-Dimensional Spectroscopy of Disordered Semiconductor Quantum Wells and Quantum Dots
Energy Technology Data Exchange (ETDEWEB)
Cundiff, Steven T. [Univ. of Colorado, Boulder, CO (United States)
2016-05-03
This final report describes the activities undertaken under grant "Optical Two-Dimensional Spectroscopy of Disordered Semiconductor Quantum Wells and Quantum Dots". The goal of this program was to implement optical 2-dimensional Fourier transform spectroscopy and apply it to electronic excitations, including excitons, in semiconductors. Specifically of interest are quantum wells that exhibit disorder due to well width fluctuations and quantum dots. In both cases, 2-D spectroscopy will provide information regarding coupling among excitonic localization sites.
Laser driven impurity states in two-dimensional quantum dots and quantum rings
Laroze, D.; Barseghyan, M.; Radu, A.; Kirakosyan, A. A.
2016-11-01
The hydrogenic donor impurity states in two-dimensional GaAs/Ga0.7Al0.3As quantum dot and quantum ring have been investigated under the action of intense laser field. A laser dressed effect on both electron confining and electron-impurity Coulomb interaction potentials has been considered. The single electron energy spectrum and wave functions have been found using the effective mass approximation and exact diagonalization technique. The accidental degeneracy of the impurity states have been observed for different positions of the impurity and versus values of the laser field parameter. The obtained theoretical results indicate a novel opportunity to tune the performance of quantum dots and quantum rings and to control their specific properties by means of laser field.
Energy Technology Data Exchange (ETDEWEB)
Nevedomskiy, V. N., E-mail: nevedom@mail.ioffe.ru; Bert, N. A.; Chaldyshev, V. V. [Russian Academy of Sciences, Ioffe Physical–Technical Institute (Russian Federation); Preobrazhernskiy, V. V.; Putyato, M. A.; Semyagin, B. R. [Russian Academy of Sciences, Institute of Semiconductor Physics, Siberian Branch (Russian Federation)
2015-12-15
A single molecular-beam epitaxy process is used to produce GaAs-based heterostructures containing two-dimensional arrays of InAs semiconductor quantum dots and AsSb metal quantum dots. The twodimensional array of AsSb metal quantum dots is formed by low-temperature epitaxy which provides a large excess of arsenic in the epitaxial GaAs layer. During the growth of subsequent layers at a higher temperature, excess arsenic forms nanoinclusions, i.e., metal quantum dots in the GaAs matrix. The two-dimensional array of such metal quantum dots is created by the δ doping of a low-temperature GaAs layer with antimony which serves as a precursor for the heterogeneous nucleation of metal quantum dots and accumulates in them with the formation of AsSb metal alloy. The two-dimensional array of InAs semiconductor quantum dots is formed via the Stranski–Krastanov mechanism at the GaAs surface. Between the arrays of metal and semiconductor quantum dots, a 3-nm-thick AlAs barrier layer is grown. The total spacing between the arrays of metal and semiconductor quantum dots is 10 nm. Electron microscopy of the structure shows that the arrangement of metal quantum dots and semiconductor quantum dots in the two-dimensional arrays is spatially correlated. The spatial correlation is apparently caused by elastic strain and stress fields produced by both AsSb metal and InAs semiconductor quantum dots in the GaAs matrix.
Song, Xiang-Xiang; Liu, Di; Mosallanejad, Vahid; You, Jie; Han, Tian-Yi; Chen, Dian-Teng; Li, Hai-Ou; Cao, Gang; Xiao, Ming; Guo, Guang-Can; Guo, Guo-Ping
2015-10-28
Two-dimensional layered materials, such as transition metal dichalcogenides (TMDCs), are promising materials for future electronics owing to their unique electronic properties. With the presence of a band gap, atomically thin gate defined quantum dots (QDs) can be achieved on TMDCs. Herein, standard semiconductor fabrication techniques are used to demonstrate quantum confined structures on WSe2 with tunnel barriers defined by electric fields, therefore eliminating the edge states induced by etching steps, which commonly appear in gapless graphene QDs. Over 40 consecutive Coulomb diamonds with a charging energy of approximately 2 meV were observed, showing the formation of a QD, which is consistent with the simulations. The size of the QD could be tuned over a factor of 2 by changing the voltages applied to the top gates. These results shed light on a way to obtain smaller quantum dots on TMDCs with the same top gate geometry compared to traditional GaAs/AlGaAs heterostructures with further research.
Reflectance measurement of two-dimensional photonic crystal nanocavities with embedded quantum dots
Stumpf, Wolfgang C; Kojima, Takanori; Fujita, Masayuki; Tanaka, Yoshinori; Noda, Susumu
2010-01-01
The spectra of two-dimensional photonic crystal slab nanocavities with embedded InAs quantum dots are measured by photoluminescence and reflectance. In comparing the spectra taken by these two different methods, consistency with the nanocavities' resonant wavelengths is found. Furthermore, it is shown that the reflectance method can measure both active and passive cavities. Q-factors of nanocavities, whose resonant wavelengths range from 1280 to 1620 nm, are measured by the reflectance method in cross polarization. Experimentally, Q-factors decrease for longer wavelengths and the intensity, reflected by the nanocavities on resonance, becomes minimal around 1360 nm. The trend of the Q-factors is explained by the change of the slab thickness relative to the resonant wavelength, showing a good agreement between theory and experiment. The trend of reflected intensity by the nanocavities on resonance can be understood as effects that originate from the PC slab and the underlying air cladding thickness. In addition...
Energy Technology Data Exchange (ETDEWEB)
Sukhanov, Aleksei A.
2017-05-15
We study the energy spectra of bound states in quantum dots (QDs) formed by an electrostatic potential in two-dimensional topological insulator (TI) and their transformation with changes in QD depth and radius. It is found that, unlike a trivial insulator, the energy difference between the levels of the ground state and first excited state can decrease with decreasing the radius and increasing the depth of the QD so that these levels intersect under some critical condition. The crossing of the levels results in unusual features of optical properties caused by intraceneter electron transitions. In particular, it leads to significant changes of light absorption due to electron transitions between such levels and to the transient electroluminescence induced by electrical tuning of QD and TI parameters. In the case of magnetic TIs, the polarization direction of the absorbed or emitted circularly polarized light is changed due to the level crossing.
Laser driven intraband optical transitions in two-dimensional quantum dots and quantum rings
Barseghyan, M. G.; Kirakosyan, A. A.; Laroze, D.
2017-01-01
The intraband optical absorption have been investigated in the presence of hydrogenic donor impurity in GaAs/GaAlAs quantum dot and quantum ring in the intense laser field. The single electron energy spectrum and wave functions have been found using the effective mass approximation and exact diagonalization technique. Different selection rules are obtained for intraband transitions depending on the direction of incident light polarization. Due to the accidental degeneracy of the laser dressed impurity states the crossings of the curves of the threshold energies and the dipole matrix elements on laser field parameter have been observed. The intraband absorption coefficient is calculated for different locations of hydrogenic donor impurity and different values of intense laser field parameter. The obtained results show that the absorption spectrum can exhibit either a blue- or redshift depending on the impurity location, values of the laser field parameter and direction of incident light polarization. The obtained theoretical results indicate a novel opportunity to tune the performance of new devices, based on the quantum dots and quantum rings and to control their specific properties by means of intense laser and hydrogenic donor impurity.
Low-Lying States of the A+B-A+B- Coulomb Systems in Two-Dimensional Quantum Dots
Institute of Scientific and Technical Information of China (English)
XIE Wen-Fang
2001-01-01
The features of the low-lying spectra of four-body A+B-A+B- systems have been deduced based on symmetry. Using the method of few-body physics, we calculate the energy spectra of A + B- A + B- systems in a harmonic quantum dot. We find that the biexciton in a two-dimensional quantum dot may have other bound excited states and the quantum mechanical symmetry plays a crucialrole in determining the energy levels and structures of the low-lying states.
Roslyak, O.; Gumbs, Godfrey; Mukamel, S.
2012-05-01
We study the localization of dressed Dirac electrons in a cylindrical quantum dot (QD) formed on monolayer and bilayer graphene by spatially different potential profiles. Short lived excitonic states which are too broad to be resolved in linear spectroscopy are revealed by cross peaks in the photon-echo nonlinear technique. Signatures of the dynamic gap in the two-dimensional spectra are discussed. The effect of the Coulomb induced exciton-exciton scattering and the formation of biexciton molecules are demonstrated.
Spin-Orbit Splitting in Semiconductor Quantum Dots with a Two-Dimensional Ring Model
Institute of Scientific and Technical Information of China (English)
FENG Jun-Sheng; LIU Zheng
2009-01-01
We present a theoretical study of the energy levels with two-dimensional ring confining potential in the presence of the Rashba spin-orbit interaction.The features of some low-lying states in various strengths of the Rashba spin-orbit interaction are investigated.The Rashba spin-orbit splitting can also be influenced by the width of the potential barrier.The computed results show that the spin-polarized electronic states can be more easily achieved in a weakly confined dot when the confinement strength for the Rashba spin-orbit interaction is larger than a critical value.
Quantum dots and etch-induced depletion of a silicon two-dimensional electron gas
Klein, L. J.; Lewis, K. L. M.; Slinker, K. A.; Goswami, Srijit; van der Weide, D. W.; Blick, R. H.; Mooney, P. M.; Chu, J. O.; Coppersmith, S. N.; Friesen, Mark; Eriksson, M. A.
2006-01-01
The controlled depletion of electrons in semiconductors is the basis for numerous devices. Reactive-ion etching provides an effective technique for fabricating both classical and quantum devices. However, Fermi-level pinning must be carefully considered in the development of small devices, such as quantum dots. Because of depletion, the electrical size of the device is reduced in comparison with its physical dimension. To investigate this issue in modulation-doped silicon single-electron transistors, we fabricate several types of devices in silicon-germanium heterostructures using two different etches, CF4 and SF6. We estimate the depletion width associated with each etch by two methods: (i) conductance measurements in etched wires of decreasing thickness (to determine the onset of depletion), and (ii) capacitance measurements of quantum dots (to estimate the size of the active region). We find that the SF6 etch causes a much smaller depletion width, making it more suitable for device fabrication.
Effective mass theory of a two-dimensional quantum dot in the presence of magnetic field
Indian Academy of Sciences (India)
Himanshu Asnani; Raghu Mahajan; Praveen Pathak; Vijay A Singh
2009-09-01
The effective mass of electrons in low-dimensional semiconductors is position-dependent. The standard kinetic energy operator of quantum mechanics for this position-dependent mass is non-Hermitian and needs to be modified. This is achieved by imposing the BenDaniel–Duke (BDD) boundary condition. We have investigated the role of this boundary condition for semiconductor quantum dots (QDs) in one, two and three dimensions. In these systems the effective mass m i inside the dot of size R is different from the mass m o outside. Hence a crucial factor in determining the electronic spectrum is the mass discontinuity factor = /} . We have proposed a novel quantum scale, , which is a dimensionless parameter proportional to 220, where 0 represents the barrier height. We show both by numerical calculations and asymptotic analysis that the ground state energy and the surface charge density, (ρ()), can be large and dependent on . We also show that the dependence of the ground state energy on the size of the dot is infraquadratic. We also study the system in the presence of magnetic field . The BDD condition introduces a magnetic length-dependent term $(\\sqrt{\\hbar /eB})$ into and hence the ground state energy. We demonstrate that the significance of BDD condition is pronounced at large and large magnetic fields. In many cases the results using the BDD condition is significantly different from the non-Hermitian treatment of the problem.
Size Effect of a Negatively Charged Exciton in a Two-Dimensional Quantum Dot
Institute of Scientific and Technical Information of China (English)
LIU Chao; XIE Wen-Fang
2009-01-01
In this paper we study a negatively charged exciton (NCE), which is trapped by a two-dimensional (2D) parabolic potential.By using matrix diagonalization techniques, the correlation energies of the low-lying states with L = O, 1, and 2 are calculated as a function of confinement strength.We find that the size effects of different states are different.This phenomenon can be explained as a hidden symmetry, which is originated purely from symmetry.Based on symmetry, the features of the low-lying states are discussed in the influence of the 2D parabolic potential well.It is found that the confinement may cause accidental degeneracies between levels with different low-excited states.It is shown that the effect of quantum confinement on the binding energy of the heavy hole is stronger than that of a light hole.
Zhukovsky, V. Ch.; Krevchik, V. D.; Semenov, M. B.; Krevchik, P. V.; Zaytsev, R. V.; Egorov, I. A.
2016-11-01
The field and temperature dependence of the probability of two-dimensional dissipative tunneling is studied in the framework of one-instanton approximation for a model double-well oscillator potential in an external electric field at finite temperature with account for the influence of two local phonon modes for quantum dots in a system of a combined atomic force and a scanning tunneling microscope. It is demonstrated that in the mode of synchronous parallel transfer of tunneling particles from the cantilever tip to the quantum dot the two local phonon modes result in the occurrence of two stable peaks in the curve of the 2D dissipative tunneling probability as a function of the field. Qualitative comparison of the theoretical curve in the limit of weak dissociation and the experimental current-voltage characteristic for quantum dots that grow from colloidal gold under a cantilever tip at the initial stage of quantum-dot formation when the quantum dot size does not exceed 10 nm is performed. It is established that one of the two stable peaks that correspond to interaction of tunneling particles with two local phonon modes in the temperature dependence of the 2D dissipative tunneling probability can be split in two, which corresponds to the tunneling channel interference mechanism. It is found that the theoretically predicted and experimentally observed mode of quantum beats occurs near the bifurcation point.
Institute of Scientific and Technical Information of China (English)
Zhai Zhi-Yuan; Li Yu-Qi; Pan Xiao-Yin
2012-01-01
We investigate the effects due to anisotropy and magnetic field interaction for a quasi-two-dimensional Boltzmann gas in an elliptical parabolic quantum dot.The specific heat is studied with varying temperature,anisotropy,and magnetic field strength.The cases without and with the inclusion of the spin Zeeman interaction are considered.
Energy Technology Data Exchange (ETDEWEB)
Nakra Mohajer, Soukaina; El Harouny, El Hassan [Laboratoire de Physique de la Matière Condensée, Département de Physique, Faculté des Sciences, Université Abdelmalek Essaadi, B.P. 2121 M’Hannech II, 93030 Tétouan (Morocco); Ibral, Asmaa [Equipe d’Optique et Electronique du Solide, Département de Physique, Faculté des Sciences, Université Chouaïb Doukkali, B. P. 20 El Jadida Principale, El Jadida (Morocco); Laboratoire d’Instrumentation, Mesure et Contrôle, Département de Physique, Faculté des Sciences, Université Chouaïb Doukkali, B. P. 20 El Jadida Principale, El Jadida (Morocco); El Khamkhami, Jamal [Laboratoire de Physique de la Matière Condensée, Département de Physique, Faculté des Sciences, Université Abdelmalek Essaadi, B.P. 2121 M’Hannech II, 93030 Tétouan (Morocco); and others
2016-09-15
Eigenvalues equation solutions of a hydrogen-like donor impurity, confined in a hemispherical quantum dot deposited on a wetting layer and capped by an insulating matrix, are determined in the framework of the effective mass approximation. Conduction band alignments at interfaces between quantum dot and surrounding materials are described by infinite height barriers. Ground and excited states energies and wave functions are determined analytically and via one-dimensional finite difference approach in case of an on-center donor. Donor impurity is then moved from center to pole of hemispherical quantum dot and eigenvalues equation is solved via Ritz variational principle, using a trial wave function where Coulomb attraction between electron and ionized donor is taken into account, and by two-dimensional finite difference approach. Numerical codes developed enable access to variations of donor total energy, binding energy, Coulomb correlation parameter, spatial extension and radial probability density with respect to hemisphere radius and impurity position inside the quantum dot.
DEFF Research Database (Denmark)
Julsgaard, Brian; Johansen, Jeppe; Stobbe, Søren
2008-01-01
We have performed time-resolved spectroscopy on InAs quantum dot ensembles in photonic crystal membranes. The influence of the photonic crystal is investigated by varying the lattice constant systematically. We observe a strong slow down of the quantum dots’ spontaneous emission rates as the two-...... the bandgap in good agreement with local density of states calculations.......We have performed time-resolved spectroscopy on InAs quantum dot ensembles in photonic crystal membranes. The influence of the photonic crystal is investigated by varying the lattice constant systematically. We observe a strong slow down of the quantum dots’ spontaneous emission rates as the two...
Distance-dependent energy transfer between CdSe/CdS quantum dots and a two-dimensional semiconductor
Energy Technology Data Exchange (ETDEWEB)
Goodfellow, Kenneth M.; Vamivakas, A. Nick, E-mail: nick.vamivakas@rochester.edu [Institute of Optics, University of Rochester, Rochester, New York 14627 (United States); Chakraborty, Chitraleema [Materials Science, University of Rochester, Rochester, New York 14627 (United States); Sowers, Kelly [Department of Chemistry, University of Rochester, Rochester, New York 14627 (United States); Waduge, Pradeep; Wanunu, Meni [Department of Physics, Northeastern University, Boston, Massachusetts 02115 (United States); Krauss, Todd [Institute of Optics, University of Rochester, Rochester, New York 14627 (United States); Department of Chemistry, University of Rochester, Rochester, New York 14627 (United States); Driscoll, Kristina [Department of Physics, Rochester Institute of Technology, Rochester, New York 14627 (United States)
2016-01-11
Atomically thin semiconductors, such as the transition metal dichalcogenides, show great potential for nanoscale photodetection, energy harvesting, and nanophotonics. Here, we investigate the efficiency of energy transfer between colloidal quantum dots with a cadmium selenide core and cadmium sulfide shell and monolayer molybdenum diselenide (MoSe{sub 2}). We show that MoSe{sub 2} effectively quenches the fluorescence of quantum dots when the two materials are in contact. We then separate the MoSe{sub 2} and quantum dots by inserting variable thickness hexagonal boron nitride (h-BN) spacers and show that the efficiency at which the MoSe{sub 2} quenches fluorescence decreases as the h-BN thickness is increased. For distances d, this trend can be modeled by a 1/d{sup 4} decay, in agreement with theory and recent studies involving graphene.
Two-dimensional quantum repeaters
Wallnöfer, J.; Zwerger, M.; Muschik, C.; Sangouard, N.; Dür, W.
2016-11-01
The endeavor to develop quantum networks gave rise to a rapidly developing field with far-reaching applications such as secure communication and the realization of distributed computing tasks. This ultimately calls for the creation of flexible multiuser structures that allow for quantum communication between arbitrary pairs of parties in the network and facilitate also multiuser applications. To address this challenge, we propose a two-dimensional quantum repeater architecture to establish long-distance entanglement shared between multiple communication partners in the presence of channel noise and imperfect local control operations. The scheme is based on the creation of self-similar multiqubit entanglement structures at growing scale, where variants of entanglement swapping and multiparty entanglement purification are combined to create high-fidelity entangled states. We show how such networks can be implemented using trapped ions in cavities.
Suárez, I; Larrue, A; Rodríguez-Cantó, P J; Almuneau, G; Abargues, R; Chirvony, V S; Martínez-Pastor, J P
2014-08-15
In this Letter, we study a new kind of organic polymer waveguide numerically and experimentally by combining an ultrathin (10-50 nm) layer of compactly packed CdSe/ZnS core/shell colloidal quantum dots (QDs) sandwiched between two cladding poly(methyl methacrylate) (PMMA) layers. When a pumping laser beam is coupled into the waveguide edge, light is mostly confined around the QD layer, improving the efficiency of excitation. Moreover, the absence of losses in the claddings allows the propagation of the pumping laser beam along the entire waveguide length; hence, a high-intensity photoluminescence (PL) is produced. Furthermore, a novel fabrication technology is developed to pattern the PMMA into ridge structures by UV lithography in order to provide additional light confinement. The sandwich-type waveguide is analyzed in comparison to a similar one formed by a PMMA film homogeneously doped by the same QDs. A 100-fold enhancement in the waveguided PL is found for the sandwich-type case due to the higher concentration of QDs inside the waveguide.
Electron correlations in quantum dots
Tipton, D L J
2001-01-01
Quantum dot structures confine electrons in a small region of space. Some properties of semiconductor quantum dots, such as the discrete energy levels and shell filling effects visible in addition spectra, have analogies to those of atoms and indeed dots are sometimes referred to as 'artificial atoms'. However, atoms and dots show some fundamental differences due to electron correlations. For real atoms, the kinetic energy of electrons dominates over their mutual Coulomb repulsion energy and for this reason the independent electron approximation works well. For quantum dots the confining potential may be shallower than that of real atoms leading to lower electron densities and a dominance of mutual Coulomb repulsion over kinetic energy. In this strongly correlated regime the independent electron picture leads to qualitatively incorrect results. This thesis concentrates on few-electron quantum dots in the strongly correlated regime both for quasi-one-dimensional and two-dimensional dots in a square confining p...
A two-dimensional spin liquid in quantum kagome ice.
Carrasquilla, Juan; Hao, Zhihao; Melko, Roger G
2015-06-22
Actively sought since the turn of the century, two-dimensional quantum spin liquids (QSLs) are exotic phases of matter where magnetic moments remain disordered even at zero temperature. Despite ongoing searches, QSLs remain elusive, due to a lack of concrete knowledge of the microscopic mechanisms that inhibit magnetic order in materials. Here we study a model for a broad class of frustrated magnetic rare-earth pyrochlore materials called quantum spin ices. When subject to an external magnetic field along the [111] crystallographic direction, the resulting interactions contain a mix of geometric frustration and quantum fluctuations in decoupled two-dimensional kagome planes. Using quantum Monte Carlo simulations, we identify a set of interactions sufficient to promote a groundstate with no magnetic long-range order, and a gap to excitations, consistent with a Z2 spin liquid phase. This suggests an experimental procedure to search for two-dimensional QSLs within a class of pyrochlore quantum spin ice materials.
Quantum entanglement in a two-dimensional ion trap
Institute of Scientific and Technical Information of China (English)
王成志; 方卯发
2003-01-01
In this paper, we investigate the quantum entanglement in a two-dimensional ion trap system. We discuss the quantum entanglement between the ion and phonons by using reduced entropy, and that between two degrees of freedom of the vibrational motion along x and y directions by using quantum relative entropy. We discuss also the influence of initial state of the system on the quantum entanglement and the relation between two entanglements in the trapped ion system.
Spin dynamics in a two-dimensional quantum gas
DEFF Research Database (Denmark)
Pedersen, Poul Lindholm; Gajdacz, Miroslav; Deuretzbacher, Frank
2014-01-01
We have investigated spin dynamics in a two-dimensional quantum gas. Through spin-changing collisions, two clouds with opposite spin orientations are spontaneously created in a Bose-Einstein condensate. After ballistic expansion, both clouds acquire ring-shaped density distributions with superimp......We have investigated spin dynamics in a two-dimensional quantum gas. Through spin-changing collisions, two clouds with opposite spin orientations are spontaneously created in a Bose-Einstein condensate. After ballistic expansion, both clouds acquire ring-shaped density distributions...
Single semiconductor quantum dots
Energy Technology Data Exchange (ETDEWEB)
Michler, Peter (ed.) [Stuttgart Univ. (Germany). Inst. fuer Halbleiteroptik und Funktionelle Grenzflaechen
2009-07-01
This book reviews recent advances in the exciting and rapidly growing field of semiconductor quantum dots via contributions from some of the most prominent researchers in the scientific community. Special focus is given to optical, quantum optical, and spin properties of single quantum dots due to their potential applications in devices operating with single electron spins and/or single photons. This includes single and coupled quantum dots in external fields, cavity-quantum electrodynamics, and single and entangled photon pair generation. Single Semiconductor Quantum Dots also addresses growth techniques to allow for a positioned nucleation of dots as well as applications of quantum dots in quantum information technologies. (orig.)
DEFF Research Database (Denmark)
Leosson, Kristjan
Semiconductor quantum dots ("solid-state atoms") are promising candidates for quantum computers and future electronic and optoelectronic devices. Quantum dots are zero-dimensional electronic systems and therefore have discrete energy levels, similar to atoms or molecules. The size distribution...... of quantum dots, however, results in a large inhomogeneous broadening of quantum dot spectra. Work on self-assembled InGaAs/GaAs quantum dots will be presented. Properties of atom-like single-dot states are investigated optically using high spatial and spectral resolution. Single-dot spectra can be used...
DEFF Research Database (Denmark)
Leosson, Kristjan
1999-01-01
Semiconductor quantum dots ("solid state atoms") are promising candidates for quantum computers and future electronic and optoelectronic devices. Quantum dots are zero-dimensional electronic systems and therefore have discrete energy levels, similar to atoms or molecules. The size distribution...... of quantum dots, however, results in a large inhomogeneous broadening of quantum dot spectra.Work on self-assembled InGaAs/GaAs quantum dots will be presented. Properties of atom-like single-dots states are investigated optically using high spatial and spectral resolution. Single-dot spectra can be used...
Non perturbative methods in two dimensional quantum field theory
Abdalla, Elcio; Rothe, Klaus D
1991-01-01
This book is a survey of methods used in the study of two-dimensional models in quantum field theory as well as applications of these theories in physics. It covers the subject since the first model, studied in the fifties, up to modern developments in string theories, and includes exact solutions, non-perturbative methods of study, and nonlinear sigma models.
Quantum skyrmions in two-dimensional chiral magnets
Takashima, Rina; Ishizuka, Hiroaki; Balents, Leon
2016-10-01
We study the quantum mechanics of magnetic skyrmions in the vicinity of the skyrmion-crystal to ferromagnet phase boundary in two-dimensional magnets. We show that the skyrmion excitation has an energy dispersion that splits into multiple bands due to the combination of magnus force and the underlying lattice. Condensation of the skyrmions can give rise to an intermediate phase between the skyrmion crystal and ferromagnet: a quantum liquid, in which skyrmions are not spatially localized. We show that the critical behavior depends on the spin size S and the topological number of the skyrmion. Experimental signatures of quantum skyrmions in inelastic neutron-scattering measurements are also discussed.
Deterministic strain-induced arrays of quantum emitters in a two-dimensional semiconductor
Branny, Artur; Kumar, Santosh; Proux, Raphaël; Gerardot, Brian D
2017-01-01
An outstanding challenge in quantum photonics is scalability, which requires positioning of single quantum emitters in a deterministic fashion. Site positioning progress has been made in established platforms including defects in diamond and self-assembled quantum dots, albeit often with compromised coherence and optical quality. The emergence of single quantum emitters in layered transition metal dichalcogenide semiconductors offers new opportunities to construct a scalable quantum architecture. Here, using nanoscale strain engineering, we deterministically achieve a two-dimensional lattice of quantum emitters in an atomically thin semiconductor. We create point-like strain perturbations in mono- and bi-layer WSe2 which locally modify the band-gap, leading to efficient funnelling of excitons towards isolated strain-tuned quantum emitters that exhibit high-purity single photon emission. We achieve near unity emitter creation probability and a mean positioning accuracy of 120±32 nm, which may be improved with further optimization of the nanopillar dimensions. PMID:28530219
Deterministic strain-induced arrays of quantum emitters in a two-dimensional semiconductor
Branny, Artur; Kumar, Santosh; Proux, Raphaël; Gerardot, Brian D.
2017-05-01
An outstanding challenge in quantum photonics is scalability, which requires positioning of single quantum emitters in a deterministic fashion. Site positioning progress has been made in established platforms including defects in diamond and self-assembled quantum dots, albeit often with compromised coherence and optical quality. The emergence of single quantum emitters in layered transition metal dichalcogenide semiconductors offers new opportunities to construct a scalable quantum architecture. Here, using nanoscale strain engineering, we deterministically achieve a two-dimensional lattice of quantum emitters in an atomically thin semiconductor. We create point-like strain perturbations in mono- and bi-layer WSe2 which locally modify the band-gap, leading to efficient funnelling of excitons towards isolated strain-tuned quantum emitters that exhibit high-purity single photon emission. We achieve near unity emitter creation probability and a mean positioning accuracy of 120+/-32 nm, which may be improved with further optimization of the nanopillar dimensions.
Multiple Potts Models Coupled to Two-Dimensional Quantum Gravity
Baillie, C F
1992-01-01
We perform Monte Carlo simulations using the Wolff cluster algorithm of {\\it multiple} $q=2,3,4$ state Potts models on dynamical phi-cubed graphs of spherical topology in order to investigate the $c>1$ region of two-dimensional quantum gravity. Contrary to naive expectation we find no obvious signs of pathological behaviour for $c>1$. We discuss the results in the light of suggestions that have been made for a modified DDK ansatz for $c>1$.
Multiple Potts models coupled to two-dimensional quantum gravity
Baillie, C. F.; Johnston, D. A.
1992-07-01
We perform Monte Carlo simulations using the Wolff cluster algorithm of multiple q=2, 3, 4 state Potts models on dynamical phi-cubed graphs of spherical topology in order to investigate the c>1 region of two-dimensional quantum gravity. Contrary to naive expectation we find no obvious signs of pathological behaviour for c>1. We discuss the results in the light of suggestions that have been made for a modified DDK ansatz for c>1.
Topological Quantum Optics in Two-Dimensional Atomic Arrays
Perczel, J.; Borregaard, J.; Chang, D. E.; Pichler, H.; Yelin, S. F.; Zoller, P.; Lukin, M. D.
2017-07-01
We demonstrate that two-dimensional atomic emitter arrays with subwavelength spacing constitute topologically protected quantum optical systems where the photon propagation is robust against large imperfections while losses associated with free space emission are strongly suppressed. Breaking time-reversal symmetry with a magnetic field results in gapped photonic bands with nontrivial Chern numbers and topologically protected, long-lived edge states. Due to the inherent nonlinearity of constituent emitters, such systems provide a platform for exploring quantum optical analogs of interacting topological systems.
Entropic Barriers for Two-Dimensional Quantum Memories
Brown, Benjamin J.; Al-Shimary, Abbas; Pachos, Jiannis K.
2014-03-01
Comprehensive no-go theorems show that information encoded over local two-dimensional topologically ordered systems cannot support macroscopic energy barriers, and hence will not maintain stable quantum information at finite temperatures for macroscopic time scales. However, it is still well motivated to study low-dimensional quantum memories due to their experimental amenability. Here we introduce a grid of defect lines to Kitaev's quantum double model where different anyonic excitations carry different masses. This setting produces a complex energy landscape which entropically suppresses the diffusion of excitations that cause logical errors. We show numerically that entropically suppressed errors give rise to superexponential inverse temperature scaling and polynomial system size scaling for small system sizes over a low-temperature regime. Curiously, these entropic effects are not present below a certain low temperature. We show that we can vary the system to modify this bound and potentially extend the described effects to zero temperature.
DEFF Research Database (Denmark)
Leosson, Kristjan
1999-01-01
of quantum dots, however, results in a large inhomogeneous broadening of quantum dot spectra.Work on self-assembled InGaAs/GaAs quantum dots will be presented. Properties of atom-like single-dots states are investigated optically using high spatial and spectral resolution. Single-dot spectra can be used......Semiconductor quantum dots ("solid state atoms") are promising candidates for quantum computers and future electronic and optoelectronic devices. Quantum dots are zero-dimensional electronic systems and therefore have discrete energy levels, similar to atoms or molecules. The size distribution...... to probe coherence times of exciton states and relaxation processes, both of which are important for future applications....
DEFF Research Database (Denmark)
Leosson, Kristjan
of quantum dots, however, results in a large inhomogeneous broadening of quantum dot spectra. Work on self-assembled InGaAs/GaAs quantum dots will be presented. Properties of atom-like single-dot states are investigated optically using high spatial and spectral resolution. Single-dot spectra can be used......Semiconductor quantum dots ("solid-state atoms") are promising candidates for quantum computers and future electronic and optoelectronic devices. Quantum dots are zero-dimensional electronic systems and therefore have discrete energy levels, similar to atoms or molecules. The size distribution...... to probe coherence times of exciton states and relaxation processes, both of which are important for future applications....
Quantum creep in a highly crystalline two-dimensional superconductor
Saito, Yu; Kasahara, Yuichi; Ye, Jianting; Iwasa, Yoshihiro; Nojima, Tsutomu
Conventional studies on quantum phase transitions, especially on superconductor-insulator or superconductor-metal-insulator transitions have been performed in deposited metallic thin films such as Bismuth or MoGe. Although the techniques of thin films deposition have been considerably improved, unintentional disorder such as impurities and deficiencies, generating the pinning centers, seems to still exist in such systems. The mechanical exfoliated highly crystalline two-dimensional material can be a good candidate to realize a less-disordered 2D superconductor with extremely weak pinning, combined with transfer method or ionic-liquid gating. We report on the quantum metal, namely, magnetic-field-induced metallic state observed in an ion-gated two-dimensional superconductor based on an ultra-highly crystalline layered band insulator, ZrNCl. We found that the superconducting state is extremely fragile against external magnetic fields; that is, zero resistance state immediately disappears, once an external magnetic field switches on. This is because the present system is relatively clean and the pinning potential is extremely weak, which cause quantum tunneling and flux flow of vortices, resulting in metallic ground state.
The XY model coupled to two-dimensional quantum gravity
Baillie, C. F.; Johnston, D. A.
1992-09-01
We perform Monte Carlo simulations using the Wolff cluster algorithm of the XY model on both fixed and dynamical phi-cubed graphs (i.e. without and with coupling to two-dimensional quantum gravity). We compare the numerical results with the theoretical expectation that the phase transition remains of KT type when the XY model is coupled to gravity. We also examine whether the universality we discovered in our earlier work on various Potts models with the same value of the central charge, c, carries over to the XY model, which has c=1.
The XY Model Coupled to Two-Dimensional Quantum Gravity
Baillie, C F; 10.1016/0370-2693(92)91037-A
2009-01-01
We perform Monte Carlo simulations using the Wolff cluster algorithm of the XY model on both fixed and dynamical phi-cubed graphs (i.e. without and with coupling to two-dimensional quantum gravity). We compare the numerical results with the theoretical expectation that the phase transition remains of KT type when the XY model is coupled to gravity. We also examine whether the universality we discovered in our earlier work on various Potts models with the same value of the central charge, $c$, carries over to the XY model, which has $c=1$.
Quantum-dot supercrystals for future nanophotonics
Baimuratov, Anvar S.; Rukhlenko, Ivan D.; Turkov, Vadim K.; Baranov, Alexander V.; Fedorov, Anatoly V.
2013-01-01
The study of supercrystals made of periodically arranged semiconductor quantum dots is essential for the advancement of emerging nanophotonics technologies. By combining the strong spatial confinement of elementary excitations inside quantum dots and exceptional design flexibility, quantum-dot supercrystals provide broad opportunities for engineering desired optical responses and developing superior light manipulation techniques on the nanoscale. Here we suggest tailoring the energy spectrum and wave functions of the supercrystals' collective excitations through the variation of different structural and material parameters. In particular, by calculating the excitonic spectra of quantum dots assembled in two-dimensional Bravais lattices we demonstrate a wide variety of spectrum transformation scenarios upon alterations in the quantum dot arrangement. This feature offers unprecedented control over the supercrystal's electromagnetic properties and enables the development of new nanophotonics materials and devices.
Spin from defects in two-dimensional quantum field theory
Novak, Sebastian
2015-01-01
We build two-dimensional quantum field theories on spin surfaces starting from theories on oriented surfaces with networks of topological defect lines and junctions. The construction uses a combinatorial description of the spin structure in terms of a triangulation equipped with extra data. The amplitude for the spin surfaces is defined to be the amplitude for the underlying oriented surface together with a defect network dual to the triangulation. Independence of the triangulation and of the other choices follows if the line defect and junctions are obtained from a Delta-separable Frobenius algebra with involutive Nakayama automorphism in the monoidal category of topological defects. For rational conformal field theory we can give a more explicit description of the defect category, and we work out two examples related to free fermions in detail: the Ising model and the so(n) WZW model at level 1.
Ultrabroadband two-quantum two-dimensional electronic spectroscopy
Gellen, Tobias A.; Bizimana, Laurie A.; Carbery, William P.; Breen, Ilana; Turner, Daniel B.
2016-08-01
A recent theoretical study proposed that two-quantum (2Q) two-dimensional (2D) electronic spectroscopy should be a background-free probe of post-Hartree-Fock electronic correlations. Testing this theoretical prediction requires an instrument capable of not only detecting multiple transitions among molecular excited states but also distinguishing molecular 2Q signals from nonresonant response. Herein we describe a 2Q 2D spectrometer with a spectral range of 300 nm that is passively phase stable and uses only beamsplitters and mirrors. We developed and implemented a dual-chopping balanced-detection method to resolve the weak molecular 2Q signals. Experiments performed on cresyl violet perchlorate and rhodamine 6G revealed distinct 2Q signals convolved with nonresonant response. Density functional theory computations helped reveal the molecular origin of these signals. The experimental and computational results demonstrate that 2Q electronic spectra can provide a singular probe of highly excited electronic states.
Crossed Andreev effects in two-dimensional quantum Hall systems
Hou, Zhe; Xing, Yanxia; Guo, Ai-Min; Sun, Qing-Feng
2016-08-01
We study the crossed Andreev effects in two-dimensional conductor/superconductor hybrid systems under a perpendicular magnetic field. Both a graphene/superconductor hybrid system and an electron gas/superconductor one are considered. It is shown that an exclusive crossed Andreev reflection, with other Andreev reflections being completely suppressed, is obtained in a high magnetic field because of the chiral edge states in the quantum Hall regime. Importantly, the exclusive crossed Andreev reflection not only holds for a wide range of system parameters, e.g., the size of system, the width of central superconductor, and the quality of coupling between the graphene and the superconductor, but also is very robust against disorder. When the applied bias is within the superconductor gap, a robust Cooper-pair splitting process with high-efficiency can be realized in this system.
Quantum magnetotransport in a modulated two-dimensional electron gas
Park, Tae-ik; Gumbs, Godfrey
1997-09-01
Quantum mechanical calculations of the magnetotransport coefficients of a modulated two-dimensional electron gas in a perpendicular magnetic field are presented using the Kubo method. The model modulation potential used is such that the effect of the steepness of the potential and its strength on the band part of the longitudinal resistivity ρxxand the Hall resistivity ρxycould be studied. In the extreme limit of a very steep potential, a two-dimensional square array of antidots is simulated. Impurity scattering is included in the self-consistent t-matrix approximation. The results show that for a strong lateral superlattice potential, ρxyis quenched in the low magnetic field regime and as the magnetic field increases there is a large negative Hall resistivity. The intensity of this negative peak is suppressed as the strength of the modulation potential is decreased. It is also shown that the height of the negative peak depends on the steepness of the potential. The longitudinal resistivity also has some interesting features. There are Aharonov-Bohm oscillations and a double peak structure which depends on both the strength of the modulation potential as well as its slope. The numerical results show that the position and intensity of the lower peak is not very sensitive to a change in the strength of the lattice potential or its steepness. However, the upper peak is greatly reduced when the lattice potential is diminished in strength. The double peak feature in ρxxand the negative peak and quenching of the Hall effect at low magnetic fields have been observed experimentally for antidots in both the quasiclassical and quantum regimes.
Energy Technology Data Exchange (ETDEWEB)
Vukmirovic, Nenad; Wang, Lin-Wang
2009-11-10
This review covers the description of the methodologies typically used for the calculation of the electronic structure of self-assembled and colloidal quantum dots. These are illustrated by the results of their application to a selected set of physical effects in quantum dots.
Criticality in Two-Dimensional Quantum Systems: Tensor Network Approach
Ran, Shi-Ju; Li, Wei; Lewenstein, Maciej; Su, Gang
2016-01-01
Determination and characterization of criticality in two-dimensional (2D) quantum many-body systems belong to the most important challenges and problems of quantum physics. In this paper we propose an efficient scheme to solve this problem by utilizing the infinite projected entangled pair state (iPEPS), and tensor network (TN) representations. We show that the criticality of a 2D state is faithfully reproduced by the ground state (dubbed as boundary state) of a one-dimensional effective Hamiltonian constructed from its iPEPS representation. We demonstrate that for a critical state the correlation length and the entanglement spectrum of the boundary state are essentially different from those of a gapped iPEPS. This provides a solid indicator that allows to identify the criticality of the 2D state. Our scheme is verified on the resonating valence bond (RVB) states on kagom\\'e and square lattices, where the boundary state of the honeycomb RVB is found to be described by a $c=1$ conformal field theory. We apply ...
An Exciton Bound to a Neutral Donor in Quantum Dots
Institute of Scientific and Technical Information of China (English)
解文方
2002-01-01
The binding energies for an exciton (X) trapped in a two-dimensional quantum dot by a neutral donor have been calculated using the method of few-body physics for the heavy hole (σ= 0.196) and the light hole (σr = 0.707).We find that the (D0, X) complex confined in a quantum dot has in general a larger binding energy than those in a two-dimensional quantum well and a three-dimensional bulk semiconductor, and the binding energy increases with the decrease of the dot radius. At dot radius R →∞, we compare our calculated result with the previous results.
Quantum holographic encoding in a two-dimensional electron gas
Energy Technology Data Exchange (ETDEWEB)
Moon, Christopher
2010-05-26
The advent of bottom-up atomic manipulation heralded a new horizon for attainable information density, as it allowed a bit of information to be represented by a single atom. The discrete spacing between atoms in condensed matter has thus set a rigid limit on the maximum possible information density. While modern technologies are still far from this scale, all theoretical downscaling of devices terminates at this spatial limit. Here, however, we break this barrier with electronic quantum encoding scaled to subatomic densities. We use atomic manipulation to first construct open nanostructures - 'molecular holograms' - which in turn concentrate information into a medium free of lattice constraints: the quantum states of a two-dimensional degenerate Fermi gas of electrons. The information embedded in the holograms is transcoded at even smaller length scales into an atomically uniform area of a copper surface, where it is densely projected into both two spatial degrees of freedom and a third holographic dimension mapped to energy. In analogy to optical volume holography, this requires precise amplitude and phase engineering of electron wavefunctions to assemble pages of information volumetrically. This data is read out by mapping the energy-resolved electron density of states with a scanning tunnelling microscope. As the projection and readout are both extremely near-field, and because we use native quantum states rather than an external beam, we are not limited by lensing or collimation and can create electronically projected objects with features as small as {approx}0.3 nm. These techniques reach unprecedented densities exceeding 20 bits/nm{sup 2} and place tens of bits into a single fermionic state.
Raffaelle, Ryne P.; Castro, Stephanie L.; Hepp, Aloysius; Bailey, Sheila G.
2002-01-01
We have been investigating the synthesis of quantum dots of CdSe, CuInS2, and CuInSe2 for use in an intermediate bandgap solar cell. We have prepared a variety of quantum dots using the typical organometallic synthesis routes pioneered by Bawendi, et. al., in the early 1990's. However, unlike previous work in this area we have also utilized single-source precursor molecules in the synthesis process. We will present XRD, TEM, SEM and EDS characterization of our initial attempts at fabricating these quantum dots. Investigation of the size distributions of these nanoparticles via laser light scattering and scanning electron microscopy will be presented. Theoretical estimates on appropriate quantum dot composition, size, and inter-dot spacing along with potential scenarios for solar cell fabrication will be discussed.
Transport through Zero-Dimensional States in a Quantum Dot
Kouwenhoven, Leo P.; Wees, Bart J. van; Harmans, Kees J.P.M.; Williamson, John G.
1990-01-01
We have studied the electron transport through zero-dimensional (0D) states. 0D states are formed when one-dimensional edge channels are confined in a quantum dot. The quantum dot is defined in a two-dimensional electron gas with a split gate technique. To allow electronic transport, connection to
Electron spin and charge in semiconductor quantum dots
Elzerman, J.M.
2004-01-01
In this thesis, the spin and charge degree of freedom of electrons in semiconductor lateral and vertical quantum dots are experimentally investigated. The lateral quantum dot devices are defined in a two-dimensional electron gas (2DEG) below the surface of a GaAs/AlGaAs heterostructure, by metallic
Wu, Jiang
2014-01-01
This book reviews recent advances in the exciting and rapidly growing field of quantum dot molecules (QDMs). It offers state-of-the-art coverage of novel techniques and connects fundamental physical properties with device design.
Güçlü, Alev Devrim; Korkusinski, Marek; Hawrylak, Pawel
2014-01-01
This book reflects the current status of theoretical and experimental research of graphene based nanostructures, in particular quantum dots, at a level accessible to young researchers, graduate students, experimentalists and theorists. It presents the current state of research of graphene quantum dots, a single or few monolayer thick islands of graphene. It introduces the reader to the electronic and optical properties of graphite, intercalated graphite and graphene, including Dirac fermions, Berry's phase associated with sublattices and valley degeneracy, covers single particle properties of
Properties of two-dimensional electron gas containing self-organized quantum antidots
Vasilyev, Yu.; Suchalkin, S.; Zundel, M.; Heisenberg, D.; Eberl, K.; von Klitzing, K.
1999-11-01
A nonuniform two-dimensional electron gas in a heterojunction with inserted self-organized electrically inactive dots (acting as antidots) has been fabricated by molecular-beam epitaxy of AlGaAs/AlInAs/GaAs layer sequences. Transport measurements give the ratio of the transport mobility to the quantum mobility less than four, which suggests that the dominant scattering at low magnetic fields is the short-range scattering from the lateral potential of the antidots. Far-infrared cyclotron resonance (CR) spectra show an absorption mode as narrow as 0.5 cm-1 at high magnetic fields associated with the high-mobility electron gas formed between the antidot islands and confined in the lateral directions. The confinement energy of 14 cm-1 is derived from the CR spectra.
Wu, Jiang
2013-01-01
The third generation of solar cells includes those based on semiconductor quantum dots. This sophisticated technology applies nanotechnology and quantum mechanics theory to enhance the performance of ordinary solar cells. Although a practical application of quantum dot solar cells has yet to be achieved, a large number of theoretical calculations and experimental studies have confirmed the potential for meeting the requirement for ultra-high conversion efficiency. In this book, high-profile scientists have contributed tutorial chapters that outline the methods used in and the results of variou
Hexagonal graphene quantum dots
Ghosh, S.
2016-12-05
We study hexagonal graphene quantum dots, using density functional theory, to obtain a quantitative description of the electronic properties and their size dependence, considering disk and ring geometries with both armchair and zigzag edges. We show that the electronic properties of quantum dots with armchair edges are more sensitive to structural details than those with zigzag edges. As functions of the inner and outer radii, we find in the case of armchair edges that the size of the band gap follows distinct branches, while in the case of zigzag edges it changes monotonically. This behaviour is further analyzed by studying the ground state wave function and explained in terms of its localisation.
Deformed oscillator algebras for two dimensional quantum superintegrable systems
Bonatsos, Dennis; Kokkotas, K D; Bonatsos, Dennis
1994-01-01
Quantum superintegrable systems in two dimensions are obtained from their classical counterparts, the quantum integrals of motion being obtained from the corresponding classical integrals by a symmetrization procedure. For each quantum superintegrable systema deformed oscillator algebra, characterized by a structure function specific for each system, is constructed, the generators of the algebra being functions of the quantum integrals of motion. The energy eigenvalues corresponding to a state with finite dimensional degeneracy can then be obtained in an economical way from solving a system of two equations satisfied by the structure function, the results being in agreement to the ones obtained from the solution of the relevant Schrodinger equation. The method shows how quantum algebraic techniques can simplify the study of quantum superintegrable systems, especially in two dimensions.
Klimov, Victor I
2010-01-01
""Soft"" Chemical Synthesis and Manipulation of Semiconductor Nanocrystals, J.A. Hollingsworth and V.I. Klimov Electronic Structure in Semiconductor Nanocrystals: Optical Experiment, D.J. NorrisFine Structure and Polarization Properties of Band-Edge Excitons in Semiconductor Nanocrystals, A.L. EfrosIntraband Spectroscopy and Dynamics of Colloidal Semiconductor Quantum Dots, P. Guyot-Sionnest, M. Shim, and C. WangMultiexciton Phenomena in Semiconductor Nanocrystals, V.I. KlimovOptical Dynamics in Single Semiconductor Quantum Do
Sapmaz, S.
2006-01-01
Low temperature electron transport measurements on individual single wall carbon nanotubes are described in this thesis. Carbon nanotubes are small hollow cylinders made entirely out of carbon atoms. At low temperatures (below ~10 K) finite length nanotubes form quantum dots. Because of its small
Sapmaz, S.
2006-01-01
Low temperature electron transport measurements on individual single wall carbon nanotubes are described in this thesis. Carbon nanotubes are small hollow cylinders made entirely out of carbon atoms. At low temperatures (below ~10 K) finite length nanotubes form quantum dots. Because of its small si
Dissipative tunneling in structures with quantum dots and quantum molecules
Dahnovsky, Yu. I.; Krevchik, V. D.; Semenov, M. B.; Yamamoto, K.; Zhukovsky, V. Ch.; Aringazin, A. K.; Kudryashov, E. I.; Mayorov, V. G.
2005-01-01
The problem of tunneling control in systems "quantum dot - quantum well" (as well as "quantum dot - quantum dot" or quantum molecule) and "quantum dot - bulk contact" is studied as a quantum tunneling with dissipation process in the semiclassical (instanton) approximation. For these systems temperature and correlation between a quantum dot radius and a quantum well width (or another quantum dot radius) are considered to be control parameters. The condition for a single electron blockade is fo...
Quasi-two-dimensional Dirac fermions and quantum magnetoresistance in LaAgBi$_2$
Wang, Kefeng; Graf, D.; Petrovic, C.
2016-01-01
We report quasi-two-dimensional Dirac fermions and quantum magnetoresistance in LaAgBi$_2$. The band structure shows several narrow bands with nearly linear energy dispersion and Dirac-cone-like points at the Fermi level. The quantum oscillation experiments revealed one quasi-two-dimensional Fermi pocket and another complex pocket with small cyclotron resonant mass. The in-plane transverse magnetoresistance exhibits a crossover at a critical field $B^*$ from semiclassical weak-field $B^2$ dep...
Two-dimensional ion trap lattice on a microchip for quantum simulation
Sterling, R C; Weidt, S; Lake, K; Srinivasan, P; Webster, S C; Kraft, M; Hensinger, W K
2013-01-01
Using a controllable quantum system it is possible to simulate other highly complex quantum systems efficiently overcoming an in-principle limitation of classical computing. Trapped ions constitute such a highly controllable quantum system. So far, no dedicated architectures for the simulation of two-dimensional spin lattices using trapped ions in radio-frequency ion traps have been produced, limiting the possibility of carrying out such quantum simulations on a large scale. We report the operation of a two-dimensional ion trap lattice integrated in a microchip capable of implementing quantum simulations of two-dimensional spin lattices. Our device provides a scalable microfabricated architecture for trapping such ion lattices with coupling strengths between neighbouring ions sufficient to provide a powerful platform for the implementation of quantum simulations. In order to realize this device we developed a specialist fabrication process that allows for the application of very large voltages. We fabricated ...
Quantum search on the two-dimensional lattice using the staggered model with Hamiltonians
Portugal, R.; Fernandes, T. D.
2017-04-01
Quantum search on the two-dimensional lattice with one marked vertex and cyclic boundary conditions is an important problem in the context of quantum algorithms with an interesting unfolding. It avails to test the ability of quantum walk models to provide efficient algorithms from the theoretical side and means to implement quantum walks in laboratories from the practical side. In this paper, we rigorously prove that the recent-proposed staggered quantum walk model provides an efficient quantum search on the two-dimensional lattice, if the reflection operators associated with the graph tessellations are used as Hamiltonians, which is an important theoretical result for validating the staggered model with Hamiltonians. Numerical results show that on the two-dimensional lattice staggered models without Hamiltonians are not as efficient as the one described in this paper and are, in fact, as slow as classical random-walk-based algorithms.
Dipolar quantum electrodynamics of the two-dimensional electron gas
Todorov, Yanko
2015-03-01
Similarly to a previous work on the homogeneous electron gas [Y. Todorov, Phys. Rev. B 89, 075115 (2014), 10.1103/PhysRevB.89.075115], we apply the Power-Zienau-Wooley (PZW) formulation of the quantum electrodynamics to the case of an electron gas quantum confined by one-dimensional potential. We provide a microscopic description of all collective plasmon modes of the gas, oscillating both along and perpendicular to the direction of quantum confinement. Furthermore, we study the interaction of the collective modes with a photonic structure, planar metallic waveguide, by using the full expansion of the electromagnetic field into normal modes. We show how the boundary conditions for the electromagnetic field influence both the transverse light-matter coupling and the longitudinal particle-particle interactions. The PZW descriptions appear thus as a convenient tool to study semiconductor quantum optics in geometries where quantum-confined particles interact with strongly confined electromagnetic fields in microresonators, such as the ones used to achieve the ultrastrong light-matter coupling regime.
Exciton-Phonon Scattering in CdSe/ZnSe Quantum Dots
Institute of Scientific and Technical Information of China (English)
张立功; 申德振; 范希武; 吕少哲
2002-01-01
A temperature-dependent photoluminescence measurement is performed in CdSe/ZnSe quantum dots with a ZnCdSe quantum well. We deduce the temperature dependence of the exciton linewidth and peak energy of the zero-dimensional exciton in the quantum dots and two-dimensional exciton in the CdSe wetting layer. The experimental data reveal a reduction of homogeneous broadening of the exciton line in the quantum dots in comparison with that in the two-dimensional wetting layer, which indicates the decrease of exciton and optical phonon coupling in the CdSe quantum dots.
Colloidal Double Quantum Dots.
Teitelboim, Ayelet; Meir, Noga; Kazes, Miri; Oron, Dan
2016-05-17
Pairs of coupled quantum dots with controlled coupling between the two potential wells serve as an extremely rich system, exhibiting a plethora of optical phenomena that do not exist in each of the isolated constituent dots. Over the past decade, coupled quantum systems have been under extensive study in the context of epitaxially grown quantum dots (QDs), but only a handful of examples have been reported with colloidal QDs. This is mostly due to the difficulties in controllably growing nanoparticles that encapsulate within them two dots separated by an energetic barrier via colloidal synthesis methods. Recent advances in colloidal synthesis methods have enabled the first clear demonstrations of colloidal double quantum dots and allowed for the first exploratory studies into their optical properties. Nevertheless, colloidal double QDs can offer an extended level of structural manipulation that allows not only for a broader range of materials to be used as compared with epitaxially grown counterparts but also for more complex control over the coupling mechanisms and coupling strength between two spatially separated quantum dots. The photophysics of these nanostructures is governed by the balance between two coupling mechanisms. The first is via dipole-dipole interactions between the two constituent components, leading to energy transfer between them. The second is associated with overlap of excited carrier wave functions, leading to charge transfer and multicarrier interactions between the two components. The magnitude of the coupling between the two subcomponents is determined by the detailed potential landscape within the nanocrystals (NCs). One of the hallmarks of double QDs is the observation of dual-color emission from a single nanoparticle, which allows for detailed spectroscopy of their properties down to the single particle level. Furthermore, rational design of the two coupled subsystems enables one to tune the emission statistics from single photon
Two-dimensional lattice gauge theories with superconducting quantum circuits
Energy Technology Data Exchange (ETDEWEB)
Marcos, D., E-mail: david.marcos@me.com [Institute for Quantum Optics and Quantum Information of the Austrian Academy of Sciences, A-6020 Innsbruck (Austria); Widmer, P. [Albert Einstein Center, Institute for Theoretical Physics, Bern University, CH-3012, Bern (Switzerland); Rico, E. [IPCMS (UMR 7504) and ISIS (UMR 7006), University of Strasbourg and CNRS, 67000 Strasbourg (France); Hafezi, M. [Joint Quantum Institute, NIST/University of Maryland, College Park 20742 (United States); Department of Electrical Engineering and Institute for Research in Electronics and Applied Physics, University of Maryland, College Park, MD 20742 (United States); Rabl, P. [Institute of Atomic and Subatomic Physics, TU Wien, Stadionallee 2, 1020 Wien (Austria); Wiese, U.-J. [Albert Einstein Center, Institute for Theoretical Physics, Bern University, CH-3012, Bern (Switzerland); Zoller, P. [Institute for Quantum Optics and Quantum Information of the Austrian Academy of Sciences, A-6020 Innsbruck (Austria); Institute for Theoretical Physics, University of Innsbruck, A-6020 Innsbruck (Austria)
2014-12-15
A quantum simulator of U(1) lattice gauge theories can be implemented with superconducting circuits. This allows the investigation of confined and deconfined phases in quantum link models, and of valence bond solid and spin liquid phases in quantum dimer models. Fractionalized confining strings and the real-time dynamics of quantum phase transitions are accessible as well. Here we show how state-of-the-art superconducting technology allows us to simulate these phenomena in relatively small circuit lattices. By exploiting the strong non-linear couplings between quantized excitations emerging when superconducting qubits are coupled, we show how to engineer gauge invariant Hamiltonians, including ring-exchange and four-body Ising interactions. We demonstrate that, despite decoherence and disorder effects, minimal circuit instances allow us to investigate properties such as the dynamics of electric flux strings, signaling confinement in gauge invariant field theories. The experimental realization of these models in larger superconducting circuits could address open questions beyond current computational capability.
Quantum vortex dynamics in two-dimensional neutral superfluids
Wang, C. -C J.; Duine, R.A.; MacDonald, A.H.
2010-01-01
We derive an effective action for the vortex-position degree of freedom in a superfluid by integrating out condensate phase- and density-fluctuation environmental modes. When the quantum dynamics of environmental fluctuations is neglected, we confirm the occurrence of the vortex Magnus force and
Parallel processing method for two-dimensional Sn transport code DOT3.5
Energy Technology Data Exchange (ETDEWEB)
Uematsu, Mikio [Toshiba Corp., Kawasaki, Kanagawa (Japan)
1998-03-01
A parallel processing method for the two-dimensional Sn transport code DOT3.5 has been developed to achieve drastic reduction of computation time. In the proposed method, parallelization is made with angular domain decomposition and/or space domain decomposition. Calculational speedup for parallel processing by angular domain decomposition is achieved by minimizing frequency of communications between processing elements. As for parallel processing by space domain decomposition, two-step rescaling method consisting of segmentwise rescaling and the ordinary pointwise rescaling have been developed to accelerate convergence, which will otherwise be degraded because of discontinuity at the segment boundaries. The developed method was examined with a Sun workstation using the PVM message-passing library, and sufficient speedup was observed. (author)
Single quantum dot nanowire photodetectors
Van Kouwen, M.P.; Van Weert, M.H.M.; Reimer, M.E.; Akopian, N.; Perinetti, U.; Algra, R.E.; Bakkers, E.P.A.M.; Kouwenhoven, L.P.; Zwiller, V.
2010-01-01
We report InP nanowire photodetectors with a single InAsP quantum dot as light absorbing element. With excitation above the InP band gap, the nanowire photodetectors are efficient (quantum efficiency of 4%). Under resonant excitation of the quantum dot, the photocurrent amplitude depends on the line
Single quantum dot nanowire photodetectors
Van Kouwen, M.P.; Van Weert, M.H.M.; Reimer, M.E.; Akopian, N.; Perinetti, U.; Algra, R.E.; Bakkers, E.P.A.M.; Kouwenhoven, L.P.; Zwiller, V.
2010-01-01
We report InP nanowire photodetectors with a single InAsP quantum dot as light absorbing element. With excitation above the InP band gap, the nanowire photodetectors are efficient (quantum efficiency of 4%). Under resonant excitation of the quantum dot, the photocurrent amplitude depends on the
Two-Dimensional Arrays of Neutral Atom Quantum Gates
2012-10-20
Isenhower, X. Zhang, A. Gill, T. Walker, M. Saffman. Deterministic entanglement of two neutral atoms via Rydberg blockade, Physical Review A, (09 2010...squeezing of atomic ensembles by multicolor quantum nondemolition measurements, Physical Review A, (02 2009): 0. doi: 10.1103/PhysRevA.79.023831 10/19/2012...collective encoding in holmium atoms, Physical Review A, (07 2008): 0. doi: 10.1103/PhysRevA.78.012336 10/19/2012 10.00 M Saffman, X L Zhang, A T
Directory of Open Access Journals (Sweden)
Mohamed Henini
2002-06-01
These sophisticated technologies for the growth of high quality epitaxial layers of compound semiconductor materials on single crystal semiconductor substrates are becoming increasingly important for the development of the semiconductor electronics industry. This article is intended to convey the flavor of the subject by focusing on the technology and applications of self-assembled quantum dots (QDs and to give an introduction to some of the essential characteristics.
Non-linear excitation of quantum emitters in two-dimensional hexagonal boron nitride
Schell, Andreas W; Takashima, Hideaki; Takeuchi, Shigeki; Aharonovich, Igor
2016-01-01
Two-photon absorption is an important non-linear process employed for high resolution bio-imaging and non-linear optics. In this work we realize two-photon excitation of a quantum emitter embedded in a two-dimensional material. We examine defects in hexagonal boron nitride and show that the emitters exhibit similar spectral and quantum properties under one-photon and two-photon excitation. Furthermore, our findings are important to deploy two-dimensional hexagonal boron nitride for quantum non-linear photonic applications.
Calculating Two-Dimensional Spectra with the Mixed Quantum-Classical Ehrenfest Method
van der Vegte, C. P.; Dijkstra, A. G.; Knoester, J.; Jansen, T. L. C.
2013-01-01
We present a mixed quantum-classical simulation approach to calculate two-dimensional spectra of coupled two-level electronic model systems. We include the change in potential energy of the classical system due to transitions in the quantum system using the Ehrenfest method. We study how this
Ge, Yingbin
2016-01-01
Hands-on exercises are designed for undergraduate physical chemistry students to derive two-dimensional quantum chemistry from scratch for the H atom and H[subscript 2] molecule, both in the ground state and excited states. By reducing the mathematical complexity of the traditional quantum chemistry teaching, these exercises can be completed…
Calculating Two-Dimensional Spectra with the Mixed Quantum-Classical Ehrenfest Method
van der Vegte, C. P.; Dijkstra, A. G.; Knoester, J.; Jansen, T. L. C.
2013-01-01
We present a mixed quantum-classical simulation approach to calculate two-dimensional spectra of coupled two-level electronic model systems. We include the change in potential energy of the classical system due to transitions in the quantum system using the Ehrenfest method. We study how this feedba
Quantum dots for quantum information technologies
2017-01-01
This book highlights the most recent developments in quantum dot spin physics and the generation of deterministic superior non-classical light states with quantum dots. In particular, it addresses single quantum dot spin manipulation, spin-photon entanglement and the generation of single-photon and entangled photon pair states with nearly ideal properties. The role of semiconductor microcavities, nanophotonic interfaces as well as quantum photonic integrated circuits is emphasized. The latest theoretical and experimental studies of phonon-dressed light matter interaction, single-dot lasing and resonance fluorescence in QD cavity systems are also provided. The book is written by the leading experts in the field.
Exact two-body solutions and quantum defect theory of two-dimensional dipolar quantum gas
Jie, Jianwen; Qi, Ran
2016-10-01
In this paper, we provide the two-body exact solutions of the two-dimensional (2D) Schrödinger equation with isotropic +/- 1/{r}3 interactions. An analytic quantum defect theory is constructed based on these solutions and it is applied to investigate the scattering properties as well as two-body bound states of an ultracold polar molecules confined in a quasi-2D geometry. Interestingly, we find that for the attractive case, the scattering resonance happens simultaneously in all partial waves, which has not been observed in other systems. The effect of this feature on the scattering phase shift across such resonances is also illustrated.
Tkach, N V; Zegrya, G G
2002-01-01
The theoretical investigation of the spectrum of electrons, holes, and excitons in the superlattice of cylindrical quantum dots with weakest coupling of quasiparticles between vertical layers of quantum dots is carried out. The calculations are fulfilled by the example of cylindrical quantum dots of beta-HgS introduced into beta-CdS as the superlattice. It is shown that electron and hole in such system form quasi-two-dimensional energy minibands, but excitons are described by the Sugano-Shinada model. The dependence of quasiparticle spectra on geometric parameters of the superlattice with cylindrical quantum dots is studied. It is shown that the position of minibands of all quasiparticles is very sensitive to variation of the quantum dot height
Barrier Li Quantum Dots in Magnetic Fields
Institute of Scientific and Technical Information of China (English)
LIUYi-Min; LIXiao-Zhu; YANWen-Hong; BAOCheng-Guang
2003-01-01
The methods for the few-body system are introduced to investigate the states of the barrier Li quantum dots (QDs) in an arbitrary strength of magnetic field. The configuration, which consists of a positive ion located on the z-axis at a distaneed from the two-dimensional QD plane (the x-y plane) and three electrons in the dot plane bound by the positive ion, is called a barrier Li center. The system, which consists of three electrons in the dot plane bound by the ion,is called a barrier Li QD. The dependence of energy of the state of the barrier Li QD on an external magnetic field B and the distance d is obtained. The angular momentum L of the ground states is found to jump not only with the variation orB but also with d.
Freely configurable quantum simulator based on a two-dimensional array of individually trapped ions
Mielenz, Manuel; Wittemer, Matthias; Hakelberg, Frederick; Schmied, Roman; Blain, Matthew; Maunz, Peter; Leibfried, Dietrich; Warring, Ulrich; Schaetz, Tobias
2015-01-01
A custom-built and precisely controlled quantum system may offer access to a fundamental understanding of another, less accessible system of interest. A universal quantum computer is currently out of reach, but an analog quantum simulator that makes the relevant observables, interactions, and states of a quantum model accessible could permit experimental insight into complex quantum dynamics that are intractable on conventional computers. Several platforms have been suggested and proof-of-principle experiments have been conducted. Here we characterise two-dimensional arrays of three ions trapped by radio-frequency fields in individually controlled harmonic wells forming equilateral triangles with side lengths 40 and 80 micrometer. In our approach, which is scalable to arbitrary two dimensional lattices, we demonstrate individual control of the electronic and motional degrees of freedom, preparation of a fiducial initial state with ion motion close to the ground state, as well as tuning of crucial couplings be...
Emergent topology and dynamical quantum phase transitions in two-dimensional closed quantum systems
Bhattacharya, Utso; Dutta, Amit
2017-07-01
Dynamical quantum phase transitions (DQPTs) manifested in the nonanalyticities in the temporal evolution of a closed quantum system generated by the time-independent final Hamiltonian, following a quench (or ramping) of a parameter of the Hamiltonian, is an emerging frontier of nonequilibrium quantum dynamics. We, here, introduce the notion of a dynamical topological order parameter (DTOP) that characterizes these DQPTs occurring in quenched (or ramped) two-dimensional closed quantum systems; this is quite a nontrivial generalization of the notion of DTOP introduced in Budich and Heyl [Phys. Rev. B 93, 085416 (2016), 10.1103/PhysRevB.93.085416] for one-dimensional situations. This DTOP is obtained from the "gauge-invariant" Pancharatnam phase extracted from the Loschmidt overlap, i.e., the modulus of the overlap between the initially prepared state and its time-evolved counterpart reached following a temporal evolution generated by the time-independent final Hamiltonian. This generic proposal is illustrated considering DQPTs occurring in the subsequent temporal evolution following a sudden quench of the staggered mass of the topological Haldane model on a hexagonal lattice where it stays fixed to zero or unity and makes a discontinuous jump between these two values at critical times at which DQPTs occur. What is remarkable is that while the topology of the equilibrium model is characterized by the Chern number, the emergent topology associated with the DQPTs is characterized by a generalized winding number.
Ma, Xuedan; Diroll, Benjamin T; Cho, Wooje; Fedin, Igor; Schaller, Richard D; Talapin, Dmitri V; Gray, Stephen K; Wiederrecht, Gary P; Gosztola, David J
2017-09-05
Quasi-two-dimensional nanoplatelets (NPLs) possess fundamentally different excitonic properties from zero-dimensional quantum dots. We study lateral size-dependent photon emission statistics and carrier dynamics of individual NPLs using second-order photon correlation (g((2))(τ)) spectroscopy and photoluminescence (PL) intensity-dependent lifetime analysis. Room-temperature radiative lifetimes of NPLs can be derived from maximum PL intensity periods in PL time traces. It first decreases with NPL lateral size and then stays constant, deviating from the electric dipole approximation. Analysis of the PL time traces further reveals that the single exciton quantum yield in NPLs decreases with NPL lateral size and increases with protecting shell thickness, indicating the importance of surface passivation on NPL emission quality. Second-order photon correlation (g((2))(τ)) studies of single NPLs show that the biexciton quantum yield is strongly dependent on the lateral size and single exciton quantum yield of the NPLs. In large NPLs with unity single exciton quantum yield, the corresponding biexciton quantum yield can reach unity. These findings reveal that by careful growth control and core-shell material engineering, NPLs can be of great potential for light amplification and integrated quantum photonic applications.
Electronic transport in two-dimensional systems in the quantum hall regime
Tarquini, Vinicio
The integer and the fractional quantum Hall effects are essential to the exploration of quantum matters characterized by topological phases. A quantum Hall system hosts one-dimensional (1D) chiral edge channels that manifest zero magnetoresistance, dissipationless due to the broken time reversal symmetry, and quantized Hall resistance vhe2 with v being the topological invariant (or Chern number). The 1-1 correspondence between the conducting gapless edge channels to the gapped incompressible bulk states is a defining character of a topological insulator (TI). Understanding this correspondence in real systems, especially the origin of its robustness (in terms of the limit of breakdown), is important both fundamentally and practically (i.e. in relation to spintronics). However, the breakdown mechanism, especially in light of the edge-bulk correlation, is still an open question. We adopt GaAs two-dimensional (2D) high-mobility hole systems confined in a 20 nm wide (100)-GaAs quantum wells and have perform transport measurement for a range of charge densities between 4 and 5 x 1010 cm -2 with a carrier mobility of 2 - 4 x 106 cm 2/V·s down to millikelvin temperatures. Systematic characterization of the 2D systems through Shubnikov-de Haas (SdH) oscillations yields an effective mass between 0.30 and 0.50me, in good agreement with the cyclotron resonance results. We then modify a regular Hall bar system into a unique anti-Hall bar geometry that provides an extra set of independent chiral edge channels without altering the topological invariant. We perform systematic measurement of quantum oscillations via chiral edges while simultaneously probing the bulk dynamics, through measuring across independent edges, in respond to the edge excitations. The edge-bulk correspondence reveals a non-equilibrium dynamical development of the incompressible bulk states that leads to a novel asymmetrical 1-0 Hall potential distribution. Moreover, probing the breakdown via inner and outer
Directory of Open Access Journals (Sweden)
Somsak Panyakeow
2010-10-01
Full Text Available Laterally close-packed quantum dots (QDs called quantum dot molecules (QDMs are grown by modified molecular beam epitaxy (MBE. Quantum dots could be aligned and cross hatched. Quantum rings (QRs created from quantum dot transformation during thin or partial capping are used as templates for the formations of bi-quantum dot molecules (Bi-QDMs and quantum dot rings (QDRs. Preferable quantum dot nanostructure for quantum computation based on quantum dot cellular automata (QCA is laterally close-packed quantum dot molecules having four quantum dots at the corners of square configuration. These four quantum dot sets are called quadra-quantum dots (QQDs. Aligned quadra-quantum dots with two electron confinements work like a wire for digital information transmission by Coulomb repulsion force, which is fast and consumes little power. Combination of quadra-quantum dots in line and their cross-over works as logic gates and memory bits. Molecular Beam Epitaxial growth technique called 'Droplet Epitaxy' has been developed for several quantum nanostructures such as quantum rings and quantum dot rings. Quantum rings are prepared by using 20 ML In-Ga (15:85 droplets deposited on a GaAs substrate at 390'C with a droplet growth rate of 1ML/s. Arsenic flux (7'8'10-6Torr is then exposed for InGaAs crystallization at 200'C for 5 min. During droplet epitaxy at a high droplet thickness and high temperature, out-diffusion from the centre of droplets occurs under anisotropic strain. This leads to quantum ring structures having non-uniform ring stripes and deep square-shaped nanoholes. Using these peculiar quantum rings as templates, four quantum dots situated at the corners of a square shape are regrown. Two of these four quantum dots are aligned either or, which are preferable crystallographic directions of quantum dot alignment in general.
Origin of the inverse energy cascade in two-dimensional quantum turbulence
Skaugen, Audun
2016-01-01
We unravel the intimate connection between fundamental characteristics of two dimensional turbulence, i.e. the large-scale coherent structures and the inverse energy cascade. We propose a driven, dissipative point vortex model that is able to capture the dynamics of two-dimensional quantum turbulence by the emergent clustering of same-sign vortices, which form a non-equilibrium analogue of Onsager vortex equilibria. The inverse energy cascade developing in a statistically neutral system originates from this clustering of co-rotating and counter-rotating vortices. The Kolmogorov energy spectrum $k^{-5/3}$ is attributed to the scale-free correlations in the vorticity field fluctuations, here measured by the weighted pair correlation function that has a power-law decay as $r^{-4/3}$ on inertial separation lengthscales $r$. This scale-invariant statistics of vorticity, attributed to a conformal symmetry of two-dimensional classical turbulence, draws further analogies between classical and quantum turbulence beyon...
Two-dimensional quantum compass model in a staggered field: some rigorous results
Institute of Scientific and Technical Information of China (English)
He Pei-Song; You Wen-Long; Tian Guang-Shan
2011-01-01
We study the properties of the two-dimensional quantum compass model in a staggered field. Using the PerronFr(o)enius theorem and the reflection positivity method, we rigorously determine the low energy spectrum of this model and its global ground state Ψ0. Furthermore, we show that Ψ0 has a directional long-range order.
Expectation value of composite field $T{\\bar T}$ in two-dimensional quantum field theory
Zamolodchikov, Alexander B.
2004-01-01
I show that the expectation value of the composite field $T{\\bar T}$, built from the components of the energy-momentum tensor, is expressed exactly through the expectation value of the energy-momentum tensor itself. The relation is derived in two-dimensional quantum field theory under broad assumptions, and does not require integrability.
Quantum computing via defect states in two-dimensional antidot lattices.
Flindt, Christian; Mortensen, Niels Asger; Jauho, Antti-Pekka
2005-12-01
We propose a new structure suitable for quantum computing in a solid-state environment: designed defect states in antidot lattices superimposed on a two-dimensional electron gas at a semiconductor heterostructure. State manipulation can be obtained with gate control. Model calculations indicate that it is feasible to fabricate structures whose energy level structure is robust against thermal dephasing.
Scaling dimensions of manifestly generally covariant operators in two-dimensional quantum gravity
Nishimura, J; Tsuchiya, A; Jun Nishimura; Shinya Tamura; Asato Tsuchiya
1994-01-01
Using (2+$\\epsilon$)-dimensional quantum gravity recently formulated by Kawai, Kitazawa and Ninomiya, we calculate the scaling dimensions of manifestly generally covariant operators in two-dimensional quantum gravity coupled to $(p,q)$ minimal conformal matter. In the spectrum appear all the scaling dimensions of the scaling operators in the matrix model except the boundary operators, while there are also many others which have no corresponding scaling dimensions in the matrix model.
Quantum dots: Rethinking the electronics
Bishnoi, Dimple
2016-05-01
In this paper, we demonstrate theoretically that the Quantum dots are quite interesting for the electronics industry. Semiconductor quantum dots (QDs) are nanometer-scale crystals, which have unique photo physical, quantum electrical properties, size-dependent optical properties, There small size means that electrons do not have to travel as far as with larger particles, thus electronic devices can operate faster. Cheaper than modern commercial solar cells while making use of a wider variety of photon energies, including "waste heat" from the sun's energy. Quantum dots can be used in tandem cells, which are multi junction photovoltaic cells or in the intermediate band setup. PbSe (lead selenide) is commonly used in quantum dot solar cells.
Bipartite entanglement entropy in massive two-dimensional quantum field theory.
Doyon, Benjamin
2009-01-23
Recently, Cardy, Castro Alvaredo, and the author obtained the first exponential correction to saturation of the bipartite entanglement entropy at large region lengths in massive two-dimensional integrable quantum field theory. It depends only on the particle content of the model, and not on the way particles scatter. Based on general analyticity arguments for form factors, we propose that this result is universal, and holds for any massive two-dimensional model (also out of integrability). We suggest a link of this result with counting pair creations far in the past.
Po, Hoi Chun; Zhou, Qi
2015-08-13
Bosons have a natural instinct to condense at zero temperature. It is a long-standing challenge to create a high-dimensional quantum liquid that does not exhibit long-range order at the ground state, as either extreme experimental parameters or sophisticated designs of microscopic Hamiltonians are required for suppressing the condensation. Here we show that synthetic gauge fields for ultracold atoms, using either the Raman scheme or shaken lattices, provide physicists a simple and practical scheme to produce a two-dimensional algebraic quantum liquid at the ground state. This quantum liquid arises at a critical Lifshitz point, where a two-dimensional quartic dispersion emerges in the momentum space, and many fundamental properties of two-dimensional bosons are changed in its proximity. Such an ideal simulator of the quantum Lifshitz model allows experimentalists to directly visualize and explore the deconfinement transition of topological excitations, an intriguing phenomenon that is difficult to access in other systems.
Quantum Hall effect in black phosphorus two-dimensional electron system.
Li, Likai; Yang, Fangyuan; Ye, Guo Jun; Zhang, Zuocheng; Zhu, Zengwei; Lou, Wenkai; Zhou, Xiaoying; Li, Liang; Watanabe, Kenji; Taniguchi, Takashi; Chang, Kai; Wang, Yayu; Chen, Xian Hui; Zhang, Yuanbo
2016-07-01
The development of new, high-quality functional materials has been at the forefront of condensed-matter research. The recent advent of two-dimensional black phosphorus has greatly enriched the materials base of two-dimensional electron systems (2DESs). Here, we report the observation of the integer quantum Hall effect in a high-quality black phosphorus 2DES. The high quality is achieved by embedding the black phosphorus 2DES in a van der Waals heterostructure close to a graphite back gate; the graphite gate screens the impurity potential in the 2DES and brings the carrier Hall mobility up to 6,000 cm(2) V(-1) s(-1). The exceptional mobility enabled us to observe the quantum Hall effect and to gain important information on the energetics of the spin-split Landau levels in black phosphorus. Our results set the stage for further study on quantum transport and device application in the ultrahigh mobility regime.
Berry phase jumps and giant nonreciprocity in Dirac quantum dots
Rodriguez-Nieva, Joaquin F.; Levitov, Leonid S.
2016-12-01
We predict that a strong nonreciprocity in the resonance spectra of Dirac quantum dots can be induced by the Berry phase. The nonreciprocity arises in relatively weak magnetic fields and is manifest in anomalously large field-induced splittings of quantum dot resonances which are degenerate at B =0 due to time-reversal symmetry. This exotic behavior, which is governed by field-induced jumps in the Berry phase of confined electronic states, is unique to quantum dots in Dirac materials and is absent in conventional quantum dots. The effect is strong for gapless Dirac particles and can overwhelm the B -induced orbital and Zeeman splittings. A finite Dirac mass suppresses the effect. The nonreciprocity, predicted for generic two-dimensional Dirac materials, is accessible through Faraday and Kerr optical rotation measurements and scanning tunneling spectroscopy.
Nonlinear low-frequency electrostatic wave dynamics in a two-dimensional quantum plasma
Energy Technology Data Exchange (ETDEWEB)
Ghosh, Samiran, E-mail: sran_g@yahoo.com [Department of Applied Mathematics, University of Calcutta, 92, Acharya Prafulla Chandra Road, Kolkata-700 009 (India); Chakrabarti, Nikhil, E-mail: nikhil.chakrabarti@saha.ac.in [Saha Institute of Nuclear Physics, 1/AF Bidhannagar, Kolkata-700064 (India)
2016-08-15
The problem of two-dimensional arbitrary amplitude low-frequency electrostatic oscillation in a quasi-neutral quantum plasma is solved exactly by elementary means. In such quantum plasmas we have treated electrons quantum mechanically and ions classically. The exact analytical solution of the nonlinear system exhibits the formation of dark and black solitons. Numerical simulation also predicts the possible periodic solution of the nonlinear system. Nonlinear analysis reveals that the system does have a bifurcation at a critical Mach number that depends on the angle of propagation of the wave. The small-amplitude limit leads to the formation of weakly nonlinear Kadomstev–Petviashvili solitons.
On Relations between One-Dimensional Quantum and Two-Dimensional Classical Spin Systems
Directory of Open Access Journals (Sweden)
J. Hutchinson
2015-01-01
Full Text Available We exploit mappings between quantum and classical systems in order to obtain a class of two-dimensional classical systems characterised by long-range interactions and with critical properties equivalent to those of the class of one-dimensional quantum systems treated by the authors in a previous publication. In particular, we use three approaches: the Trotter-Suzuki mapping, the method of coherent states, and a calculation based on commuting the quantum Hamiltonian with the transfer matrix of a classical system. This enables us to establish universality of certain critical phenomena by extension from the results in the companion paper for the classical systems identified.
Energy Spectra of Vortex Distributions in Two-Dimensional Quantum Turbulence
Directory of Open Access Journals (Sweden)
Ashton S. Bradley
2012-10-01
Full Text Available We theoretically explore key concepts of two-dimensional turbulence in a homogeneous compressible superfluid described by a dissipative two-dimensional Gross-Pitaeveskii equation. Such a fluid supports quantized vortices that have a size characterized by the healing length ξ. We show that, for the divergence-free portion of the superfluid velocity field, the kinetic-energy spectrum over wave number k may be decomposed into an ultraviolet regime (k≫ξ^{-1} having a universal k^{-3} scaling arising from the vortex core structure, and an infrared regime (k≪ξ^{-1} with a spectrum that arises purely from the configuration of the vortices. The Novikov power-law distribution of intervortex distances with exponent -1/3 for vortices of the same sign of circulation leads to an infrared kinetic-energy spectrum with a Kolmogorov k^{-5/3} power law, which is consistent with the existence of an inertial range. The presence of these k^{-3} and k^{-5/3} power laws, together with the constraint of continuity at the smallest configurational scale k≈ξ^{-1}, allows us to derive a new analytical expression for the Kolmogorov constant that we test against a numerical simulation of a forced homogeneous, compressible, two-dimensional superfluid. The numerical simulation corroborates our analysis of the spectral features of the kinetic-energy distribution, once we introduce the concept of a clustered fraction consisting of the fraction of vortices that have the same sign of circulation as their nearest neighboring vortices. Our analysis presents a new approach to understanding two-dimensional quantum turbulence and interpreting similarities and differences with classical two-dimensional turbulence, and suggests new methods to characterize vortex turbulence in two-dimensional quantum fluids via vortex position and circulation measurements.
Barroso, Margarida M
2011-03-01
Quantum dots are semiconductor nanocrystals that have broad excitation spectra, narrow emission spectra, tunable emission peaks, long fluorescence lifetimes, negligible photobleaching, and ability to be conjugated to proteins, making them excellent probes for bioimaging applications. Here the author reviews the advantages and disadvantages of using quantum dots in bioimaging applications, such as single-particle tracking and fluorescence resonance energy transfer, to study receptor-mediated transport.
Hydrophobin-Encapsulated Quantum Dots.
Taniguchi, Shohei; Sandiford, Lydia; Cooper, Maggie; Rosca, Elena V; Ahmad Khanbeigi, Raha; Fairclough, Simon M; Thanou, Maya; Dailey, Lea Ann; Wohlleben, Wendel; von Vacano, Bernhard; de Rosales, Rafael T M; Dobson, Peter J; Owen, Dylan M; Green, Mark
2016-02-01
The phase transfer of quantum dots to water is an important aspect of preparing nanomaterials that are suitable for biological applications, and although numerous reports describe ligand exchange, very few describe efficient ligand encapsulation techniques. In this report, we not only report a new method of phase transferring quantum dots (QDs) using an amphiphilic protein (hydrophobin) but also describe the advantages of using a biological molecule with available functional groups and their use in imaging cancer cells in vivo and other imaging applications.
Barroso, Margarida M.
2011-01-01
Quantum dots are semiconductor nanocrystals that have broad excitation spectra, narrow emission spectra, tunable emission peaks, long fluorescence lifetimes, negligible photobleaching, and ability to be conjugated to proteins, making them excellent probes for bioimaging applications. Here the author reviews the advantages and disadvantages of using quantum dots in bioimaging applications, such as single-particle tracking and fluorescence resonance energy transfer, to study receptor-mediated t...
Suppression of low-frequency charge noise in gates-defined GaAs quantum dots
Energy Technology Data Exchange (ETDEWEB)
You, Jie; Li, Hai-Ou, E-mail: haiouli@ustc.edu.cn, E-mail: gpguo@ustc.edu.cn; Wang, Ke; Cao, Gang; Song, Xiang-Xiang; Xiao, Ming; Guo, Guo-Ping, E-mail: haiouli@ustc.edu.cn, E-mail: gpguo@ustc.edu.cn [Key Laboratory of Quantum Information, Chinese Academy of Sciences, University of Science and Technology of China, Hefei, Anhui 230026 (China); Synergetic Innovation Center of Quantum Information and Quantum Physics, University of Science and Technology of China, Hefei, Anhui 230026 (China)
2015-12-07
To reduce the charge noise of a modulation-doped GaAs/AlGaAs quantum dot, we have fabricated shallow-etched GaAs/AlGaAs quantum dots using the wet-etching method to study the effects of two-dimensional electron gas (2DEG) underneath the metallic gates. The low-frequency 1/f noise in the Coulomb blockade region of the shallow-etched quantum dot is compared with a non-etched quantum dot on the same wafer. The average values of the gate noise are approximately 0.5 μeV in the shallow-etched quantum dot and 3 μeV in the regular quantum dot. Our results show the quantum dot low-frequency charge noise can be suppressed by the removal of the 2DEG underneath the metallic gates, which provides an architecture for noise reduction.
Interactions of a Charged Particle with Parallel Two-Dimensional Quantum Electron Gases
Institute of Scientific and Technical Information of China (English)
LI Chun-Zhi; SONG Yuan-Hong; WANG You-Nian
2008-01-01
@@ By using the linearized quantum hydrodynamic (QHD) theory, electronic excitations induced by a charged particle moving between or over two parallel two-dimensional quantum electron gases (2DQEG) are investigated. The calculation shows that the influence of the quantum effects on the interaction process should be taken into account. Including the quantum statistical and quantum diffraction effects, the general expressions of the induced potential and the stopping power are obtained. Our simulation results indicate that a V-shaped oscillatory wake potential exists in the electron gases during the test charge intrusion. Meanwhile, double peaks will occur in the stopping power when the distance of two surfaces is smaller and the test charge gets closer to any one of the two sheets.
Wenzel, Sandro; Bogacz, Leszek; Janke, Wolfhard
2008-09-19
The two-dimensional J-J' dimerized quantum Heisenberg model is studied on the square lattice by means of (stochastic series expansion) quantum Monte Carlo simulations as a function of the coupling ratio alpha=J'/J. The critical point of the order-disorder quantum phase transition in the J-J' model is determined as alpha_c=2.5196(2) by finite-size scaling for up to approximately 10 000 quantum spins. By comparing six dimerized models we show, contrary to the current belief, that the critical exponents of the J-J' model are not in agreement with the three-dimensional classical Heisenberg universality class. This lends support to the notion of nontrivial critical excitations at the quantum critical point.
Ultraviolet finiteness of Chiral Perturbation Theory for two-dimensional Quantum Electrodynamics
Paston, S A; Franke, V A
2003-01-01
We consider the perturbation theory in the fermion mass (chiral perturbation theory) for the two-dimensional quantum electrodynamics. With this aim, we rewrite the theory in the equivalent bosonic form in which the interaction is exponential and the fermion mass becomes the coupling constant. We reformulate the bosonic perturbation theory in the superpropagator language and analyze its ultraviolet behavior. We show that the boson Green's functions without vacuum loops remain finite in all orders of the perturbation theory in the fermion mass.
Quantum Monte Carlo simulation of a two-dimensional Majorana lattice model
Hayata, Tomoya; Yamamoto, Arata
2017-07-01
We study interacting Majorana fermions in two dimensions as a low-energy effective model of a vortex lattice in two-dimensional time-reversal-invariant topological superconductors. For that purpose, we implement ab initio quantum Monte Carlo simulation to the Majorana fermion system in which the path-integral measure is given by a semipositive Pfaffian. We discuss spontaneous breaking of time-reversal symmetry at finite temperatures.
Fabrication of quantum-dot devices in graphene
Directory of Open Access Journals (Sweden)
Satoshi Moriyama, Yoshifumi Morita, Eiichiro Watanabe, Daiju Tsuya, Shinya Uji, Maki Shimizu and Koji Ishibashi
2010-01-01
Full Text Available We describe our recent experimental results on the fabrication of quantum-dot devices in a graphene-based two-dimensional system. Graphene samples were prepared by micromechanical cleavage of graphite crystals on a SiO2/Si substrate. We performed micro-Raman spectroscopy measurements to determine the number of layers of graphene flakes during the device fabrication process. By applying a nanofabrication process to the identified graphene flakes, we prepared a double-quantum-dot device structure comprising two lateral quantum dots coupled in series. Measurements of low-temperature electrical transport show the device to be a series-coupled double-dot system with varied interdot tunnel coupling, the strength of which changes continuously and non-monotonically as a function of gate voltage.
Gopinath, T; Kumar, Anil
2006-12-01
Hadamard spectroscopy has earlier been used to speed-up multi-dimensional NMR experiments. In this work, we speed-up the two-dimensional quantum computing scheme, by using Hadamard spectroscopy in the indirect dimension, resulting in a scheme which is faster and requires the Fourier transformation only in the direct dimension. Two and three qubit quantum gates are implemented with an extra observer qubit. We also use one-dimensional Hadamard spectroscopy for binary information storage by spatial encoding and implementation of a parallel search algorithm.
Quantum spin-glass transition in the two-dimensional electron gas
Indian Academy of Sciences (India)
Subir Sachdev
2002-02-01
We discuss the possibility of spin-glass order in the vicinity of the unexpected metallic state of the two-dimensional electron gas in zero applied magnetic ﬁeld. An average ferromagnetic moment may also be present, and the spin-glass order then resides in the plane orthogonal to the ferromagnetic moment. We argue that a quantum transition involving the destruction of the spin-glass order in an applied in-plane magnetic ﬁeld offers a natural explanation of some features of recent magnetoconductance measurements. We present a quantum ﬁeld theory for such a transition and compute its mean ﬁeld properties.
Unconventional critical activated scaling of two-dimensional quantum spin glasses
Matoz-Fernandez, D. A.; Romá, F.
2016-07-01
We study the critical behavior of two-dimensional short-range quantum spin glasses by numerical simulations. Using a parallel tempering algorithm, we calculate the Binder cumulant for the Ising spin glass in a transverse magnetic field with two different short-range bond distributions, the bimodal and the Gaussian ones. Through an exhaustive finite-size analysis, we show that the cumulant probably follows an unconventional activated scaling, which we interpret as new evidence supporting the hypothesis that the quantum critical behavior is governed by an infinite randomness fixed point.
Two-dimensional distributed-phase-reference protocol for quantum key distribution
DEFF Research Database (Denmark)
Bacco, Davide; Christensen, Jesper Bjerge; Usuga Castaneda, Mario A.;
2016-01-01
Quantum key distribution (QKD) and quantum communication enable the secure exchange of information between remote parties. Currently, the distributed-phase-reference (DPR) protocols, which are based on weak coherent pulses, are among the most practical solutions for long-range QKD. During the last...... 10 years, long-distance fiber-based DPR systems have been successfully demonstrated, although fundamental obstacles such as intrinsic channel losses limit their performance. Here, we introduce the first two-dimensional DPR-QKD protocol in which information is encoded in the time and phase of weak...
Gerard, Valerie; Govan, Joseph; Loudon, Alexander; Baranov, Alexander V.; Fedorov, Anatoly V.; Gun'ko, Yurii K.
2015-10-01
The main goal of our research is to develop new types of technologically important optically active quantum dot (QD) based materials, study their properties and explore their biological applications. For the first time chiral II-VI QDs have been prepared by us using microwave induced heating with the racemic (Rac), D- and L-enantiomeric forms of penicillamine as stabilisers. Circular dichroism (CD) studies of these QDs have shown that D- and L-penicillamine stabilised particles produced mirror image CD spectra, while the particles prepared with a Rac mixture showed only a weak signal. It was also demonstrated that these QDs show very broad emission bands between 400 and 700 nm due to defects or trap states on the surfaces of the nanocrystals. These QDs have demonstrated highly specific chiral recognition of various biological species including aminoacids. The utilisation of chiral stabilisers also allowed the preparation of new water soluble white emitting CdS nano-tetrapods, which demonstrated circular dichroism in the band-edge region of the spectrum. Biological testing of chiral CdS nanotetrapods displayed a chiral bias for an uptake of the D- penicillamine stabilised nano-tetrapods by cancer cells. It is expected that this research will open new horizons in the chemistry of chiral nanomaterials and their application in nanobiotechnology, medicine and optical chemo- and bio-sensing.
Three-body recombination in a quasi-two-dimensional quantum gas
Huang, Bo; Zenesini, Alessandro; Grimm, Rudolf
2016-05-01
Quantum three-body recombination in three-dimensional systems is influenced by a series of weakly bound trimers known as Efimov states, which are induced by short-range interactions and exhibit a discrete scaling symmetry. On the other hand, two-dimensional systems with contact interactions are characterized by continuous scale invariance and support no Efimov physics. This raises questions about the behaviour of three-body recombination in the transition from three to two dimensions. We use ultracold caesium atoms trapped in anisotropic potentials formed by a pair of counter-propagating laser beams to experimentally investigate three-body recombination in quasi-two-dimensional systems with tunable confinement and tunable interactions. In our recent experiments, we observed a smooth transition of the three-body recombination rate coefficient from a three-dimensional to a deeply quasi-two-dimensional system. A comparison between the results obtained near two Feshbach resonances indicates a universal behaviour of three-body recombination in the quasi-two-dimensional regime. Austrian Science Fund FWF within project P23106.
Suzuki, Nozomu; Wang, Yichun; Elvati, Paolo; Qu, Zhi-Bei; Kim, Kyoungwon; Jiang, Shuang; Baumeister, Elizabeth; Lee, Jaewook; Yeom, Bongjun; Bahng, Joong Hwan; Lee, Jaebeom; Violi, Angela; Kotov, Nicholas A
2016-02-23
Chiral nanostructures from metals and semiconductors attract wide interest as components for polarization-enabled optoelectronic devices. Similarly to other fields of nanotechnology, graphene-based materials can greatly enrich physical and chemical phenomena associated with optical and electronic properties of chiral nanostructures and facilitate their applications in biology as well as other areas. Here, we report that covalent attachment of l/d-cysteine moieties to the edges of graphene quantum dots (GQDs) leads to their helical buckling due to chiral interactions at the "crowded" edges. Circular dichroism (CD) spectra of the GQDs revealed bands at ca. 210-220 and 250-265 nm that changed their signs for different chirality of the cysteine edge ligands. The high-energy chiroptical peaks at 210-220 nm correspond to the hybridized molecular orbitals involving the chiral center of amino acids and atoms of graphene edges. Diverse experimental and modeling data, including density functional theory calculations of CD spectra with probabilistic distribution of GQD isomers, indicate that the band at 250-265 nm originates from the three-dimensional twisting of the graphene sheet and can be attributed to the chiral excitonic transitions. The positive and negative low-energy CD bands correspond to the left and right helicity of GQDs, respectively. Exposure of liver HepG2 cells to L/D-GQDs reveals their general biocompatibility and a noticeable difference in the toxicity of the stereoisomers. Molecular dynamics simulations demonstrated that d-GQDs have a stronger tendency to accumulate within the cellular membrane than L-GQDs. Emergence of nanoscale chirality in GQDs decorated with biomolecules is expected to be a general stereochemical phenomenon for flexible sheets of nanomaterials.
Extraordinary behaviors in a two-dimensional decoherent alternative quantum walk
Chen, Tian; Zhang, Xiangdong
2016-07-01
We reveal the quantum and classical behaviors of the two-dimensional (2D) alternative quantum walk (AQW) in the presence of decoherence. For different kinds of decoherence, the analytic expressions for the moments of position distribution of the AQW are obtained. Taking the broken line noise and coin decoherence as examples of decoherence, we find that when decoherence emerges in only one direction, the anisotropic position distribution pattern appears, and not all the motions of the walker exhibit the transition from quantum to classical behaviors. Considering the effect of decoherence, we reveal the anisotropic correlations between the x (y ) position of the 2D walker and the state of the coin in 2D AQWs.
Tunable band topology reflected by fractional quantum Hall States in two-dimensional lattices.
Wang, Dong; Liu, Zhao; Cao, Junpeng; Fan, Heng
2013-11-01
Two-dimensional lattice models subjected to an external effective magnetic field can form nontrivial band topologies characterized by nonzero integer band Chern numbers. In this Letter, we investigate such a lattice model originating from the Hofstadter model and demonstrate that the band topology transitions can be realized by simply introducing tunable longer-range hopping. The rich phase diagram of band Chern numbers is obtained for the simple rational flux density and a classification of phases is presented. In the presence of interactions, the existence of fractional quantum Hall states in both |C| = 1 and |C| > 1 bands is confirmed, which can reflect the band topologies in different phases. In contrast, when our model reduces to a one-dimensional lattice, the ground states are crucially different from fractional quantum Hall states. Our results may provide insights into the study of new fractional quantum Hall states and experimental realizations of various topological phases in optical lattices.
Levanony, Dana
2010-01-01
We study the internal structure of a two-dimensional dilatonic evaporating black hole, based on the CGHS model. At the semiclassical level, a (weak) spacelike singularity was previously found to develop inside the black hole. We employ here a simplified quantum formulation of spacetime dynamics in the neighborhood of this singularity, using a minisuperspace-like approach. Quantum evolution is found to be regular and well-defined at the semiclassical singularity. A well-localized initial wave-packet propagating towards the singularity bounces off the latter and retains its well-localized form. Our simplified quantum treatment thus suggests that spacetime may extend semiclassically beyond the singularity, and also signifies the specific extension.
Mesoscopic Cavity Quantum Electrodynamics with Quantum Dots
Childress, L I; Lukin, M D
2003-01-01
We describe an electrodynamic mechanism for coherent, quantum mechanical coupling between spacially separated quantum dots on a microchip. The technique is based on capacitive interactions between the electron charge and a superconducting transmission line resonator, and is closely related to atomic cavity quantum electrodynamics. We investigate several potential applications of this technique which have varying degrees of complexity. In particular, we demonstrate that this mechanism allows design and investigation of an on-chip double-dot microscopic maser. Moreover, the interaction may be extended to couple spatially separated electron spin states while only virtually populating fast-decaying superpositions of charge states. This represents an effective, controllable long-range interaction, which may facilitate implementation of quantum information processing with electron spin qubits and potentially allow coupling to other quantum systems such as atomic or superconducting qubits.
Quantum-dot emitters in photonic nanostructures
DEFF Research Database (Denmark)
Hvam, Jørn Märcher; Stobbe, Søren; Lodahl, Peter
2010-01-01
The spontaneous emission from self-assembled semiconductor quantum dots is strongly influenced by the environment in which they are placed. This can be used to determine fundamental optical properties of the quantum dots as well as to manipulate and control the quantum-dot emission itself....
Beer's law in semiconductor quantum dots
Adamashvili, G T
2010-01-01
The propagation of a coherent optical linear wave in an ensemble of semiconductor quantum dots is considered. It is shown that a distribution of transition dipole moments of the quantum dots changes significantly the polarization and Beer's absorption length of the ensemble of quantum dots. Explicit analytical expressions for these quantities are presented.
Evidence of two-dimensional quantum Wigner Crystal in a zero magnetic field
Huang, Jian; Pfeiffer, Loren; West, Ken
2014-03-01
In disorder-dominated cases, Anderson localization occurs as a result of destructive interference effects caused by (short-ranged) random disorders. On the other hand, in interaction-dominated scenarios, striking manifestations of quantum physics emerge in response to strong inter-particle Coulomb energy (EC). The most prominent interaction-driven effect is the Wigner crystallization (WC) of electrons, an electron solid made up with spatially separated charges settling in a form of a lattice. The classical version of the crystallization, with the Debye temperature ΘD
Test of quantum thermalization in the two-dimensional transverse-field Ising model
Blaß, Benjamin; Rieger, Heiko
2016-12-01
We study the quantum relaxation of the two-dimensional transverse-field Ising model after global quenches with a real-time variational Monte Carlo method and address the question whether this non-integrable, two-dimensional system thermalizes or not. We consider both interaction quenches in the paramagnetic phase and field quenches in the ferromagnetic phase and compare the time-averaged probability distributions of non-conserved quantities like magnetization and correlation functions to the thermal distributions according to the canonical Gibbs ensemble obtained with quantum Monte Carlo simulations at temperatures defined by the excess energy in the system. We find that the occurrence of thermalization crucially depends on the quench parameters: While after the interaction quenches in the paramagnetic phase thermalization can be observed, our results for the field quenches in the ferromagnetic phase show clear deviations from the thermal system. These deviations increase with the quench strength and become especially clear comparing the shape of the thermal and the time-averaged distributions, the latter ones indicating that the system does not completely lose the memory of its initial state even for strong quenches. We discuss our results with respect to a recently formulated theorem on generalized thermalization in quantum systems.
Nanoscale quantum-dot supercrystals
Baimuratov, Anvar S.; Turkov, Vadim K.; Rukhlenko, Ivan D.; Baranov, Alexander V.; Fedorov, Anatoly V.
2013-09-01
We develop a theory allowing one to calculate the energy spectra and wave functions of collective excitations in twoand three-dimensional quantum-dot supercrystals. We derive analytical expressions for the energy spectra of twodimensional supercrystals with different Bravias lattices, and use them to analyze the possibility of engineering the supercrystals' band structure. We demonstrate that the variation of the supercrystal's parameters (such as the symmetry of the periodic lattice and the properties of the quantum dots or their environment) enables an unprecedented control over its optical properties, thus paving a way towards the development of new nanophotonics materials.
Quantum State Transfer in a Two-dimensional Regular Spin Lattice of Triangular Shape
Miki, Hiroshi; Vinet, Luc; Zhedanov, Alexei
2012-01-01
Quantum state transfer in a triangular domain of a two-dimensional, equally-spaced, spin lat- tice with non-homogeneous nearest-neighbor couplings is analyzed. An exact solution of the one- excitation dynamics is provided in terms of 2-variable Krawtchouk orthogonal polynomials that have been recently defined. The probability amplitude for an excitation to transit from one site to another is given. For some values of the parameters, perfect transfer is shown to take place from the apex of the lattice to the boundary hypotenuse.
Modeling A.C. Electronic Transport through a Two-Dimensional Quantum Point Contact
Energy Technology Data Exchange (ETDEWEB)
Aronov, I.E.; Beletskii, N.N.; Berman, G.P.; Campbell, D.K.; Doolen, G.D.; Dudiy, S.V.
1998-12-07
We present the results on the a.c. transport of electrons moving through a two-dimensional (2D) semiconductor quantum point contact (QPC). We concentrate our attention on the characteristic properties of the high frequency admittance ({omega}{approximately}0 - 50 GHz), and on the oscillations of the admittance in the vicinity of the separatrix (when a channel opens or closes), in presence of the relaxation effects. The experimental verification of such oscillations in the admittance would be a strong confirmation of the semi-classical approach to the a.c. transport in a QPC, in the separatrix region.
Institute of Scientific and Technical Information of China (English)
JI An-Chun; TIAN Guang-Shan
2006-01-01
In the present paper, we calculate the Gaussian correction to the critical value Jc⊥ caused by quantum spin fluctuation in a two-dimensional spatially anisotropic Heisenberg antiferromagnet with integer spin S. Previously, someauthors computed this quantity by the mean-field theory based on the Schwinger boson representation of spin operators.However, for S = 1, their result is much less than the one derived by numerical calculations. By taking the effect ofquantum spin fluctuation into consideration, we are able to produce a greatly improved result.
Chen, Y. F.; Tung, J. C.; Tuan, P. H.; Yu, Y. T.; Liang, H. C.; Huang, K. F.
2017-01-01
A general method is developed to characterize the family of classical periodic orbits from the quantum Green's function for the two-dimensional (2D) integrable systems. A decomposing formula related to the beta function is derived to link the quantum Green's function with the individual classical periodic orbits. The practicality of the developed formula is demonstrated by numerically analyzing the 2D commensurate harmonic oscillators and integrable quantum billiards. Numerical analyses reveal that the emergence of the classical features in quantum Green's functions principally comes from the superposition of the degenerate states for 2D harmonic oscillators. On the other hand, the damping factor in quantum Green's functions plays a critical role to display the classical features in mesoscopic regime for integrable quantum billiards, where the physical function of the damping factor is to lead to the coherent superposition of the nearly degenerate eigenstates.
Nonequilibrium Phase Transition in a Two-Dimensional Driven Open Quantum System
Directory of Open Access Journals (Sweden)
G. Dagvadorj
2015-11-01
Full Text Available The Berezinskii-Kosterlitz-Thouless mechanism, in which a phase transition is mediated by the proliferation of topological defects, governs the critical behavior of a wide range of equilibrium two-dimensional systems with a continuous symmetry, ranging from spin systems to superconducting thin films and two-dimensional Bose fluids, such as liquid helium and ultracold atoms. We show here that this phenomenon is not restricted to thermal equilibrium, rather it survives more generally in a dissipative highly nonequilibrium system driven into a steady state. By considering a quantum fluid of polaritons of an experimentally relevant size, in the so-called optical parametric oscillator regime, we demonstrate that it indeed undergoes a phase transition associated with a vortex binding-unbinding mechanism. Yet, the exponent of the power-law decay of the first-order correlation function in the (algebraically ordered phase can exceed the equilibrium upper limit: this shows that the ordered phase of driven-dissipative systems can sustain a higher level of collective excitations before the order is destroyed by topological defects. Our work suggests that the macroscopic coherence phenomena, observed recently in interacting two-dimensional light-matter systems, result from a nonequilibrium phase transition of the Berezinskii-Kosterlitz-Thouless rather than the Bose-Einstein condensation type.
Electron nuclear spin transfer in quantum-dot networks
Prada, M.; Toonen, R. C.; Blick, R. H.; Harrison, P.
2005-05-01
We investigate the conductance spectra of coupled quantum dots to study systematically the nuclear spin relaxation of different geometries of a two-dimensional network of quantum dots and observe spin blockade dependence on the electronic configurations. We derive the conductance using the Beenakker approach generalized to an array of quantum dots where we consider the nuclear spin transfer to electrons by hyperfine coupling. This allows us to predict the relevant memory effects on the different electronic states by studying the evolution of the single electron resonances in the presence of nuclear spin relaxation. We find that the gradual depolarization of the nuclear system is imprinted in the conductance spectra of the multidot system. Our calculations of the temporal evolution of the conductance resonance reveal that spin blockade can be lifted by hyperfine coupling.
Broadband room temperature strong coupling between quantum dots and metamaterials.
Indukuri, Chaitanya; Yadav, Ravindra Kumar; Basu, J K
2017-08-17
Herein, we report the first demonstration of room temperature enhanced light-matter coupling in the visible regime for metamaterials using cooperative coupled quasi two dimensional quantum dot assemblies located at precise distances from the hyperbolic metamaterial (HMM) templates. The non-monotonic variation of the magnitude of strong coupling, manifested in terms of strong splitting of the photoluminescence of quantum dots, can be explained in terms of enhanced LDOS near the surface of such metamaterials as well as the plasmon mediated super-radiance of closely spaced quantum dots (QDs). Our methodology of enhancing broadband, room temperature, light-matter coupling in the visible regime for metamaterials opens up new possibilities of utilising these materials for a wide range of applications including QD based thresholdless nanolasers and novel metamaterial based integrated photonic devices.
Charge transport and localization in atomically coherent quantum dot solids
Whitham, Kevin; Yang, Jun; Savitzky, Benjamin H.; Kourkoutis, Lena F.; Wise, Frank; Hanrath, Tobias
2016-05-01
Epitaxial attachment of quantum dots into ordered superlattices enables the synthesis of quasi-two-dimensional materials that theoretically exhibit features such as Dirac cones and topological states, and have major potential for unprecedented optoelectronic devices. Initial studies found that disorder in these structures causes localization of electrons within a few lattice constants, and highlight the critical need for precise structural characterization and systematic assessment of the effects of disorder on transport. Here we fabricated superlattices with the quantum dots registered to within a single atomic bond length (limited by the polydispersity of the quantum dot building blocks), but missing a fraction (20%) of the epitaxial connections. Calculations of the electronic structure including the measured disorder account for the electron localization inferred from transport measurements. The calculations also show that improvement of the epitaxial connections will lead to completely delocalized electrons and may enable the observation of the remarkable properties predicted for these materials.
Spin storage in quantum dot ensembles and single quantum dots
Energy Technology Data Exchange (ETDEWEB)
Heiss, Dominik
2009-10-15
This thesis deals with the investigation of spin relaxation of electrons and holes in small ensembles of self-assembled quantum dots using optical techniques. Furthermore, a method to detect the spin orientation in a single quantum dot was developed in the framework of this thesis. A spin storage device was used to optically generate oriented electron spins in small frequency selected quantum dot ensembles using circularly polarized optical excitation. The spin orientation can be determined by the polarization of the time delayed electroluminescence signal generated by the device after a continuously variable storage time. The degree of spin polarized initialization was found to be limited to 0.6 at high magnetic fields, where anisotropic effects are compensated. The spin relaxation was directly measured as a function of magnetic field, lattice temperature and s-shell transition energy of the quantum dot by varying the spin storage time up to 30 ms. Very long spin lifetimes are obtained with a lower limit of T{sub 1}=20 ms at B=4 T and T=1 K. A strong magnetic field dependence T{sub 1}{proportional_to}B{sup -5} has been observed for low temperatures of T=1 K which weakens as the temperature is increased. In addition, the temperature dependence has been determined with T{sub 1}{proportional_to}T{sup -1}. The characteristic dependencies on magnetic field and temperature lead to the identification of the spin relaxation mechanism, which is governed by spin-orbit coupling and mediated by single phonon scattering. This finding is qualitatively supported by the energy dependent measurements. The investigations were extended to a modified device design that enabled studying the spin relaxation dynamics of heavy holes in self-assembled quantum dots. The measurements show a polarization memory effect for holes with up to 0.1 degree of polarization. Furthermore, investigations of the time dynamics of the hole spin relaxation reveal surprisingly long lifetimes T{sub 1}{sup h
Numerical study for the c-dependence of fractal dimension in two-dimensional quantum gravity
Kawamoto, N; Kawamoto, Noboru; Yotsuji, Kenji
2002-01-01
We numerically investigate the fractal structure of two-dimensional quantum gravity coupled to matter central charge c for $-2 \\leq c \\leq 1$. We reformulate Q-state Potts model into the model which can be identified as a weighted percolation cluster model and can make continuous change of Q, which relates c, on the dynamically triangulated lattice. The c-dependence of the critical coupling is measured from the percolation probability and susceptibility. The c-dependence of the string susceptibility of the quantum surface is evaluated and has very good agreement with the theoretical predictions. The c-dependence of the fractal dimension based on the finite size scaling hypothesis is measured and has excellent agreement with one of the theoretical predictions previously proposed except for the region near $c\\approx 1$.
Huard; Cox; Saminadayar; Arnoult; Tatarenko
2000-01-01
The dependence of the optical absorption spectrum of a semiconductor quantum well on two-dimensional electron concentration n(e) is studied using CdTe samples. The trion peak (X-) seen at low n(e) evolves smoothly into the Fermi edge singularity at high n(e). The exciton peak (X) moves off to high energy, weakens, and disappears. The X,X- splitting is linear in n(e) and closely equal to the Fermi energy plus the trion binding energy. For Cd0.998Mn0.002Te quantum wells in a magnetic field, the X,X- splitting reflects unequal Fermi energies for M = +/-1/2 electrons. The data are explained by Hawrylak's theory of the many-body optical response including spin effects.
Kallin, Ann B; Hyatt, Katharine; Singh, Rajiv R P; Melko, Roger G
2013-03-29
We develop a method to calculate the bipartite entanglement entropy of quantum models, in the thermodynamic limit, using a numerical linked-cluster expansion (NLCE) involving only rectangular clusters. It is based on exact diagonalization of all n×m rectangular clusters at the interface between entangled subsystems A and B. We use it to obtain the Renyi entanglement entropy of the two-dimensional transverse field Ising model, for arbitrary real Renyi index α. Extrapolating these results as a function of the order of the calculation, we obtain universal pieces of the entanglement entropy associated with lines and corners at the quantum critical point. They show NLCE to be one of the few methods capable of accurately calculating universal properties of arbitrary Renyi entropies at higher dimensional critical points.
Two-dimensional distributed-phase-reference protocol for quantum key distribution
Bacco, Davide; Christensen, Jesper Bjerge; Castaneda, Mario A. Usuga; Ding, Yunhong; Forchhammer, Søren; Rottwitt, Karsten; Oxenløwe, Leif Katsuo
2016-12-01
Quantum key distribution (QKD) and quantum communication enable the secure exchange of information between remote parties. Currently, the distributed-phase-reference (DPR) protocols, which are based on weak coherent pulses, are among the most practical solutions for long-range QKD. During the last 10 years, long-distance fiber-based DPR systems have been successfully demonstrated, although fundamental obstacles such as intrinsic channel losses limit their performance. Here, we introduce the first two-dimensional DPR-QKD protocol in which information is encoded in the time and phase of weak coherent pulses. The ability of extracting two bits of information per detection event, enables a higher secret key rate in specific realistic network scenarios. Moreover, despite the use of more dimensions, the proposed protocol remains simple, practical, and fully integrable.
Cavity quantum electrodynamics with many-body states of a two-dimensional electron gas.
Smolka, Stephan; Wuester, Wolf; Haupt, Florian; Faelt, Stefan; Wegscheider, Werner; Imamoglu, Ataç
2014-10-17
Light-matter interaction has played a central role in understanding as well as engineering new states of matter. Reversible coupling of excitons and photons enabled groundbreaking results in condensation and superfluidity of nonequilibrium quasiparticles with a photonic component. We investigated such cavity-polaritons in the presence of a high-mobility two-dimensional electron gas, exhibiting strongly correlated phases. When the cavity was on resonance with the Fermi level, we observed previously unknown many-body physics associated with a dynamical hole-scattering potential. In finite magnetic fields, polaritons show distinct signatures of integer and fractional quantum Hall ground states. Our results lay the groundwork for probing nonequilibrium dynamics of quantum Hall states and exploiting the electron density dependence of polariton splitting so as to obtain ultrastrong optical nonlinearities.
Erlingsson, S.I.
2003-01-01
The main theme of this thesis is the hyperfine interaction between the many lattice nuclear spins and electron spins localized in GaAs quantum dots. This interaction is an intrinsic property of the material. Despite the fact that this interaction is rather weak, it can, as shown in this thesis, stro
Colloidal quantum dot solar cells
Sargent, Edward H.
2012-03-01
Solar cells based on solution-processed semiconductor nanoparticles -- colloidal quantum dots -- have seen rapid advances in recent years. By offering full-spectrum solar harvesting, these cells are poised to address the urgent need for low-cost, high-efficiency photovoltaics.
Tomczak, Nikodem; Liu, Rongrong; Vancso, Julius G.
2013-01-01
Quantum Dots (QDs) are semiconductor nanocrystals with distinct photophysical properties finding applications in biology, biosensing, and optoelectronics. Polymeric coatings of QDs are used primarily to provide long-term colloidal stability to QDs dispersed in solutions and also as a source of addit
Tunable few-electron double quantum dots with integrated charge read-out
Elzerman, J. M.; Hanson, R.; Greidanus, J. S.; Willems van Beveren, L. H.; De Franceschi, S.; Vandersypen, L. M. K.; Tarucha, S.; Kouwenhoven, L. P.
2004-11-01
We report on the realization of few-electron double quantum dots defined in a two-dimensional electron gas by means of surface gates on top of a GaAs/AlGaAs heterostructure. Two quantum point contacts (QPCs) are placed in the vicinity of the double quantum dot and serve as charge detectors. These enable determination of the number of conduction electrons on each dot. This number can be reduced to zero, while still allowing transport measurements through the double dot. The coupling between the two dots can be controlled even in the few-electron regime. Microwave radiation is used to pump an electron from one dot to the other by absorption of a single photon. The experiments demonstrate that this quantum dot circuit can serve as a good starting point for a scalable spin-qubit system.
Coherent control of quantum dots
DEFF Research Database (Denmark)
Johansen, Jeppe; Lodahl, Peter; Hvam, Jørn Märcher
In recent years much effort has been devoted to the use of semiconductor quantum dotsystems as building blocks for solid-state-based quantum logic devices. One importantparameter for such devices is the coherence time, which determines the number ofpossible quantum operations. From earlier...... measurements the coherence time of the selfassembledquantum dots (QDs) has been reported to be limited by the spontaneousemission rate at cryogenic temperatures1.In this project we propose to alter the coherence time of QDs by taking advantage of arecent technique on modifying spontaneous emission rates...
Semiconductor double quantum dot micromaser.
Liu, Y-Y; Stehlik, J; Eichler, C; Gullans, M J; Taylor, J M; Petta, J R
2015-01-16
The coherent generation of light, from masers to lasers, relies upon the specific structure of the individual emitters that lead to gain. Devices operating as lasers in the few-emitter limit provide opportunities for understanding quantum coherent phenomena, from terahertz sources to quantum communication. Here we demonstrate a maser that is driven by single-electron tunneling events. Semiconductor double quantum dots (DQDs) serve as a gain medium and are placed inside a high-quality factor microwave cavity. We verify maser action by comparing the statistics of the emitted microwave field above and below the maser threshold. Copyright © 2015, American Association for the Advancement of Science.
Coherent control of quantum dots
DEFF Research Database (Denmark)
Johansen, Jeppe; Lodahl, Peter; Hvam, Jørn Märcher
In recent years much effort has been devoted to the use of semiconductor quantum dotsystems as building blocks for solid-state-based quantum logic devices. One importantparameter for such devices is the coherence time, which determines the number ofpossible quantum operations. From earlier...... measurements the coherence time of the selfassembledquantum dots (QDs) has been reported to be limited by the spontaneousemission rate at cryogenic temperatures1.In this project we propose to alter the coherence time of QDs by taking advantage of arecent technique on modifying spontaneous emission rates...
Brightness-equalized quantum dots
Lim, Sung Jun; Zahid, Mohammad U.; Le, Phuong; Ma, Liang; Entenberg, David; Harney, Allison S.; Condeelis, John; Smith, Andrew M.
2015-10-01
As molecular labels for cells and tissues, fluorescent probes have shaped our understanding of biological structures and processes. However, their capacity for quantitative analysis is limited because photon emission rates from multicolour fluorophores are dissimilar, unstable and often unpredictable, which obscures correlations between measured fluorescence and molecular concentration. Here we introduce a new class of light-emitting quantum dots with tunable and equalized fluorescence brightness across a broad range of colours. The key feature is independent tunability of emission wavelength, extinction coefficient and quantum yield through distinct structural domains in the nanocrystal. Precise tuning eliminates a 100-fold red-to-green brightness mismatch of size-tuned quantum dots at the ensemble and single-particle levels, which substantially improves quantitative imaging accuracy in biological tissue. We anticipate that these materials engineering principles will vastly expand the optical engineering landscape of fluorescent probes, facilitate quantitative multicolour imaging in living tissue and improve colour tuning in light-emitting devices.
Phase diagram and correlation functions of the two-dimensional dissipative quantum XY model
Hou, Changtao; Varma, Chandra M.
2016-11-01
The two-dimensional quantum XY model, with a Caldeira-Leggett form of dissipation, is applicable to the quantum-critical properties of diverse experimental systems, ranging from superconductor to insulator transitions, ferromagnetic and antiferromagnetic transitions in metals, to the loop-current order transition in cuprates. We solve the reexpression of this model in terms of orthogonal topological excitations, vortices, and a variety of instantons, by renormalization group methods. The calculations explain the extraordinary properties of the model discovered in Monte Carlo calculations: the product form of the quantum-critical fluctuations in space and time, a spatial correlation length proportional to the logarithm of the temporal correlation length near the transition from a disordered to a fully ordered state, and the occurrence of a phase with spatial order without temporal order. They are intimately related to the flow of the metric of time in relation to the metric of space, i.e., of the dynamical critical exponent z . These properties appear to be essential in understanding the strange metallic phase found in a variety of quantum-critical transitions as well as the accompanying high-temperature superconductivity.
Spin dynamics and magnetic correlation length in two-dimensional quantum heisenberg antiferromagnets
Carretta; Ciabattoni; Cuccoli; Mognaschi; Rigamonti; Tognetti; Verrucchi
2000-01-10
The correlated spin dynamics and temperature dependence of the correlation length xi(T) in two-dimensional quantum (S = 1/2) Heisenberg antiferromagnets (2DQHAF) on a square lattice are discussed in light of experimental results of proton spin lattice relaxation in copper formiate tetradeuterate. In this compound the exchange constant is much smaller than the one in recently studied 2DQHAF, such as La2CuO4 and Sr2CuO2Cl2. Thus the spin dynamics can be probed in detail over a wider temperature range. The NMR relaxation rates turn out to be in excellent agreement with a theoretical mode-coupling calculation. The deduced temperature behavior of xi(T) is in agreement with high-temperature expansions, quantum Monte Carlo simulations, and the pure quantum self-consistent harmonic approximation. Contrary to the predictions of the theories based on the nonlinear sigma model, no evidence of crossover between different quantum regimes is observed.
Colloidal quantum dots: synthesis, properties and applications
Brichkin, S. B.; Razumov, V. F.
2016-12-01
Key recent results obtained in studies of a new class of luminophores, colloidal quantum dots, are analyzed. Modern methods for the synthesis and post-synthetic treatment of colloidal quantum dots that make it possible to achieve record high quantum yield of luminescence and to modify their characteristics for specific applications are considered. Currently important avenues of research on colloidal quantum dots and the problems in and prospects for their practical applications in various fields are discussed. The bibliography includes 272 references.
Quantum Computer Using Coupled Quantum Dot Molecules
Wu, N J; Natori, A; Yasunaga, H; Wu*, Nan-Jian
1999-01-01
We propose a method for implementation of a quantum computer using artificial molecules. The artificial molecule consists of two coupled quantum dots stacked along z direction and one single electron. One-qubit and two-qubit gates are constructed by one molecule and two coupled molecules, respectively.The ground state and the first excited state of the molecule are used to encode the |0> and |1> states of a qubit. The qubit is manipulated by a resonant electromagnetic wave that is applied directly to the qubit through a microstrip line. The coupling between two qubits in a quantum controlled NOT gate is switched on (off) by floating (grounding) the metal film electrodes. We study the operations of the gates by using a box-shaped quantum dot model and numerically solving a time-dependent Schridinger equation, and demonstrate that the quantum gates can perform the quantum computation. The operating speed of the gates is about one operation per 4ps. The reading operation of the output of the quantum computer can...
Three Quantum Dots Embedded in Aharonov-Bohm Rings
Toonen, Ryan; Hãttel, Andreas; Goswami, Srijit; Eberl, Karl; Eriksson, Mark; van der Weide, Daniel; Blick, Robert
2004-03-01
Coherent coupling of two quantum dots embedded in a ring-geometry has been demonstrated by Holleitner et al.(A.W. Holleitner, H. Qin, C.R. Decker, K. Eberl, and R.H. Blick, phCoherent Coupling of Two Quantum Dots Embedded in an Aharonov-Bohm Ring), Phys. Rev. Lett. 87, 256802 (2001) Recording of the Aharonov-Bohm oscillations in such a circuit has proven that the phases of electron wave functions can be manipulated directly. We have since enhanced the complexity of this system by embedding three quantum dots in such a ring-geometry. As before, our quantum dots are formed by laterally constricting a two-dimensional electron gas (2DEG) in an Al_xGa_1-xAs/GaAs heterostructure. The new, essential ingredient of this experiment is an additional third port--added to the ring for individually addressing the third quantum dot. This circuit allows us to investigate phenomena associated with phase-switching between separate ports. We will discuss first results and give a simple model of circuit operation.
Shabani, Javad
2016-10-01
Theory suggests that the interface between a one-dimensional semiconductor (Sm) with strong spin-orbit coupling and a superconductor (S) hosts Majorana modes with nontrivial topological properties. A key challenge in fabrication of such hybrid devices is forming highly transparent contacts between the active electrons in the semiconductor and the superconducting metal. Recently, it has been shown that a near perfect interface and a highly transparent contact can be achieved using epitaxial growth of aluminum on InAs nanowires. In this work, we present the first two-dimensional epitaxial superconductor-semiconductor material system that can serve as a platform for topological superconductivity. We show that our material system, Al-InAs, satisfies all the requirements necessary to reach into the topological superconducting regime by individual characterization of the semiconductor two dimensional electron system, superconductivity of Al and performance of S-Sm-S junctions. This exciting development might lead to a number of useful applications ranging from spintronics to quantum computing.
Thermoelectric energy harvesting with quantum dots.
Sothmann, Björn; Sánchez, Rafael; Jordan, Andrew N
2015-01-21
We review recent theoretical work on thermoelectric energy harvesting in multi-terminal quantum-dot setups. We first discuss several examples of nanoscale heat engines based on Coulomb-coupled conductors. In particular, we focus on quantum dots in the Coulomb-blockade regime, chaotic cavities and resonant tunneling through quantum dots and wells. We then turn toward quantum-dot heat engines that are driven by bosonic degrees of freedom such as phonons, magnons and microwave photons. These systems provide interesting connections to spin caloritronics and circuit quantum electrodynamics.
Multifarious topological quantum phase transitions in two-dimensional topological superconductors
Liu, Xiao-Ping; Zhou, Yuan; Wang, Yi-Fei; Gong, Chang-De
2016-06-01
We study the two-dimensional topological superconductors of spinless fermions in a checkerboard-lattice Chern-insulator model. With the short-range p-wave superconducting pairing, multifarious topological quantum phase transitions have been found and several phases with high Chern numbers have been observed. We have established a rich phase diagram for these topological superconducting states. A finite-size checkerboard-lattice cylinder with a harmonic trap potential has been further investigated. Based upon the self-consistent numerical calculations of the Bogoliubov-de Gennes equations, various phase transitions have also been identified at different regions of the system. Multiple pairs of Majorana fermions are found to be well-separated and localized at the phase boundaries between the phases characterized by different Chern numbers.
Theory of the vortex-clustering transition in a confined two-dimensional quantum fluid
Yu, Xiaoquan; Nian, Jun; Reeves, Matthew T; Bradley, Ashton S
2016-01-01
Clustering of like-sign vortices in a planar bounded domain is known to occur at negative temperature, a phenomenon that Onsager demonstrated to be a consequence of bounded phase space. In a confined superfluid, quantized vortices can support such an ordered phase, provided they evolve as an almost isolated subsystem containing sufficient energy. A detailed theoretical understanding of the statistical mechanics of such states thus requires a microcanonical approach. Here we develop an analytical theory of the vortex clustering transition in a neutral system of quantum vortices confined to a two-dimensional disk geometry, within the microcanonical ensemble. As the system energy increases above a critical value, the system develops global order via the emergence of a macroscopic dipole structure from the homogeneous phase of vortices, spontaneously breaking the Z2 symmetry associated with invariance under vortex circulation exchange, and the rotational SO(2) symmetry due to the disk geometry. The dipole structu...
One- and Two-Dimensional Nuclear Magnetic Resonance Spectroscopy with a Diamond Quantum Sensor
Boss, J. M.; Chang, K.; Armijo, J.; Cujia, K.; Rosskopf, T.; Maze, J. R.; Degen, C. L.
2016-05-01
We report on Fourier spectroscopy experiments performed with near-surface nitrogen-vacancy centers in a diamond chip. By detecting the free precession of nuclear spins rather than applying a multipulse quantum sensing protocol, we are able to unambiguously identify the NMR species devoid of harmonics. We further show that, by engineering different Hamiltonians during free precession, the hyperfine coupling parameters as well as the nuclear Larmor frequency can be selectively measured with up to five digits of precision. The protocols can be combined to demonstrate two-dimensional Fourier spectroscopy. Presented techniques will be useful for mapping nuclear coordinates in molecules deposited on diamond sensor chips, en route to imaging their atomic structure.
Magnetoelectronic transport of the two-dimensional electron gas in CdSe single quantum wells
Indian Academy of Sciences (India)
P K Ghosh; A Ghosal; D Chattopadhyay
2009-02-01
Hall mobility and magnetoresistance coefficient for the two-dimensional (2D) electron transport parallel to the heterojunction interfaces in a single quantum well of CdSe are calculated with a numerical iterative technique in the framework of Fermi–Dirac statistics. Lattice scatterings due to polar-mode longitudinal optic (LO) phonons, and acoustic phonons via deformation potential and piezoelectric couplings, are considered together with background and remote ionized impurity interactions. The parallel mode of piezoelectric scattering is found to contribute more than the perpendicular mode. We observe that the Hall mobility decreases with increasing temperature but increases with increasing channel width. The magnetoresistance coefficient is found to decrease with increasing temperature and increase with increasing magnetic field in the classical region.
Donor-bound electron states in a two-dimensional quantum ring under uniform magnetic field
Institute of Scientific and Technical Information of China (English)
Jia Bo-Yong; Yu Zhong-Yuan; Liu Yu-Min; Han Li-Hong; Yao Wen-Jie; Feng Hao; Ye Han
2011-01-01
The electron states in a two-dimensional GaAs/AlGaAs quantum ring are theoretically studied in effective mass approximation. On-centre donor impurity and uniform magnetic field perpendicular to the ring plane are taken into account. The energy spectrum with different angular momentum changes dramatically with the geometry of the ring.The donor impurity reduces the energies with an almost fixed value; however, the magnetic field alters energies in a more complex way. For example, energy levels under magnetic field will cross each other when increasing the inner radius and outer radius of the ring, leading to the fact that the arrangement of energy levels is distinct in certain geometry of the ring. Moreover, energy levels with negative angular momentum exhibit the non-monotonous dependence on the increasing magnetic field.
Unbinding of mutually avoiding random walks and two-dimensional quantum gravity
Carlon, Enrico; Baiesi, Marco
2004-12-01
We analyze the unbinding transition for a two-dimensional lattice polymer in which the constituent strands are mutually avoiding random walks. At low temperatures the strands are bound and form a single self-avoiding walk. We show that unbinding in this model is a strong first order transition. The entropic exponents associated with denaturated loops and end-segment distributions show sharp differences at the transition point and in the high temperature phase. Their values can be deduced from some exact arguments relying on a conformal mapping of copolymer networks into a fluctuating geometry, i.e., in the presence of quantum gravity. An excellent agreement between analytical and numerical estimates is observed for all cases analyzed.
Quantum Phase Transition in the Two-Dimensional Random Transverse-Field Ising Model
Pich, C.; Young, A. P.
1998-03-01
We study the quantum phase transition in the random transverse-field Ising model by Monte Carlo simulations. In one-dimension it has been established that this system has the following striking behavior: (i) the dynamical exponent is infinite, and (ii) the exponents for the divergence of the average and typical correlation lengths are different. An important issue is whether this behavior is special to one-dimension or whether similar behavior persists in higher dimensions. Here we attempt to answer this question by studies of the two-dimensional model. Our simulations use the Wolff cluster algorithm and the results are analyzed by anisotropic finite size scaling, paying particular attention to the Binder ratio of moments of the order parameter distribution and the distribution of the spin-spin correlation functions for various distances.
Multifarious topological quantum phase transitions in two-dimensional topological superconductors
Liu, Xiao-Ping; Zhou, Yuan; Wang, Yi-Fei; Gong, Chang-De
2016-01-01
We study the two-dimensional topological superconductors of spinless fermions in a checkerboard-lattice Chern-insulator model. With the short-range p-wave superconducting pairing, multifarious topological quantum phase transitions have been found and several phases with high Chern numbers have been observed. We have established a rich phase diagram for these topological superconducting states. A finite-size checkerboard-lattice cylinder with a harmonic trap potential has been further investigated. Based upon the self-consistent numerical calculations of the Bogoliubov-de Gennes equations, various phase transitions have also been identified at different regions of the system. Multiple pairs of Majorana fermions are found to be well-separated and localized at the phase boundaries between the phases characterized by different Chern numbers. PMID:27329219
Measurement of the quantum capacitance of two-dimensional vanadium dioxide films
Wu, Zhe; Knighton, Talbot; Tarquini, Vinicio; Huang, Jian; Sepúlveda, Nelson; Department of Physics; Astronomy, Wayne State University Collaboration; Department of Electrical; Computer Engineering, Michigan State University Collaboration
2015-03-01
With a homebuilt ac bridge, we have performed capacitance measurement of quasi two-dimensional vanadium dioxide films grown on silicon-dioxide/p-doped silicon substrate. The out-phase-signal, which corresponds to the resistivity variation, is superior to the four-terminal measurement result of the temperature dependence of the resistivity which varies by four orders of magnitude from 360K to 310K. The hysteretic behavior shows an overlap of two distinctive features that indicate a shifted structural transition relative to the Mott transition. In addition, the quantum capacitance is obtained through the in-phase signals so that d μ/dn, the inverse of the density of states, is determined as a function of temperature. This has resulted in a diverging compressibility below the critical temperature by four orders of magnitude, consistent with a Mott transition influenced by Peierls transition.
Two-dimensional topological crystalline insulator phase in quantum wells of trivial insulators
Niu, Chengwang; Buhl, Patrick M.; Bihlmayer, Gustav; Wortmann, Daniel; Blügel, Stefan; Mokrousov, Yuriy
2016-06-01
The realization of two-dimensional (2D) topological insulators (TIs) in HgTe/CdTe quantum wells (QWs) has generated an explosion of research on TIs and novel topologically nontrivial phases. Here we predict, based on first-principles calculations, that the newly discovered 2D topological crystalline insulators (TCIs) phase exists even in the QWs of trivial insulators, e.g. (Sn/Pb)Te and Na(Cl/Br), with mirror Chern number {n}{{M}}=-2. Tunable nontrivial energy gaps ranging from 4 to 238 meV are obtained, guaranteeing further room-temperature observations and applications. The combined effect of strain and electrostatic interaction that can be engineered by the cladding layers leads to a band inversion, resulting in the phase transition from trivial insulator to 2D TCIs. Our work provides a new strategy for engineering topological states in 2D materials.
Two-dimensional quantum percolation with binary non-zero hopping integrals
Dillon Thomas, Brianna; Nakanishi, Hisao
In a previous work [Dillon and Nakanishi, Eur.Phys.J B 87, 286 (2014)], we calculated the transmission coefficient of the two-dimensional quantum percolation problem and mapped out in detail the three regimes of localization, i.e., exponentially localized, power-law localized, and delocalized which had been proposed earlier [Islam and Nakanishi, Phys.Rev. E 77, 061109 (2008)]. We now consider a variation on quantum percolation in which the hopping integral (Vdiluted) associated with bonds that connect to at least one diluted site is non-zero but a fraction of the hopping integral (Vfull=1) between non-diluted sites. We study the latter model by calculating quantities such as the transmission coefficient and the inverse participation ratio and find the original quantum percolation results to be stable over a wide range of energy. In particular, except in the immediate neighborhood of the band center (where increasing Vdiluted to just 0.02*Vfull appears to eliminate localization effects), increasing Vdiluted only shifts the boundaries between the 3 regimes but does not eliminate them until the Vdiluted reaches 20
Ultrafast spectroscopy of quantum dots
Foo, E
2001-01-01
exchange-correlation interactions among the confined carriers inside the dots are suggested to be responsible. A density functional calculation for BGR of the ground state transition shows good agreement with our experimental results, especially in the high dot occupancy regime. Many-particle state scattering gives rise to large homogeneous spectral broadening of the PL peaks, from which an intradot relaxation time approx 300 fs is estimated. This observation supports the results obtained by direct excitation of carriers within the QDs. Femtosecond time-resolved photoluminescence measured by frequency up-conversion has been used to investigate carrier dynamics in InAs/GaAs self-assembled quantum dots (QDs). Our results reveal ultrafast carrier relaxation and sequential state filling. Carrier relaxation is proposed to occur by Auger-type processes, and the sequential state filling suggests that intradot relaxation is much faster than carrier capture from the InAs wetting layer. Measurements obtained by direct ...
Photon-assisted tunneling in an asymmetrically coupled triple quantum dot
Energy Technology Data Exchange (ETDEWEB)
Wang, Bao-Chuan; Cao, Gang, E-mail: gcao@ustc.edu.cn; Chen, Bao-Bao; Yu, Guo-Dong; Li, Hai-Ou; Xiao, Ming; Guo, Guo-Ping, E-mail: gpguo@ustc.edu.cn [Key Laboratory of Quantum Information, CAS, University of Science and Technology of China, Hefei, Anhui 230026 (China); Synergetic Innovation Center of Quantum Information and Quantum Physics, University of Science and Technology of China, Hefei, Anhui 230026 (China)
2016-08-14
The gate-defined quantum dot is regarded as one of the basic structures required for scalable semiconductor quantum processors. Here, we demonstrate a structure that contains three quantum dots scaled in series. The electron number of each dot and the tunnel coupling between them can be tuned conveniently using splitting gates. We tune the quantum dot array asymmetrically such that the tunnel coupling between the right dot and the central dot is much larger than that between the left dot and the central dot. When driven by microwaves, the sidebands of the photon-assisted tunneling process appear not only in the left-to-central dot transition region but also in the left-to-right dot transition region. These sidebands are both attributed to the left-to-central transition for asymmetric coupling. Our result shows that there is a region of a triple quantum dot structure that remains indistinct when studied with a normal two-dimensional charge stability diagram; this will be helpful in future studies of the scalability of quantum dot systems.
Semiconductor quantum-dot lasers and amplifiers
DEFF Research Database (Denmark)
Hvam, Jørn Märcher; Borri, Paola; Ledentsov, N. N.
2002-01-01
We have produced GaAs-based quantum-dot edge-emitting lasers operating at 1.16 mu m with record-low transparency current, high output power, and high internal quantum efficiencies. We have also realized GaAs-based quantum-dot lasers emitting at 1.3 mu m, both high-power edge emitters and low...
Semiconductor quantum dots for electron spin qubits
van der Wiel, Wilfred Gerard; Stopa, M.; Kodera, T.; Hatano, T.; Tarucha, S.
2006-01-01
We report on our recent progress in applying semiconductor quantum dots for spin-based quantum computation, as proposed by Loss and DiVincenzo (1998 Phys. Rev. A 57 120). For the purpose of single-electron spin resonance, we study different types of single quantum dot devices that are designed for
Few-electron quantum dot circuit with integrated charge read out
Elzerman, J. M.; Hanson, R.; Greidanus, J. S.; Willems van Beveren, L. H.; de Franceschi, S.; Vandersypen, L. M.; Tarucha, S.; Kouwenhoven, L. P.
2003-04-01
We report on the realization of a few-electron double quantum dot defined in a two-dimensional electron gas by means of surface gates on top of a GaAs/AlGaAs heterostructure. Two quantum point contacts are placed in the vicinity of the double quantum dot and serve as charge detectors. These enable determination of the number of conduction electrons on each dot. This number can be reduced to zero, while still allowing transport measurements through the double dot. Microwave radiation is used to pump an electron from one dot to the other by absorption of a single photon. The experiments demonstrate that this quantum dot circuit can serve as a good starting point for a scalable spin-qubit system.
Ultrasmall colloidal PbS quantum dots
Energy Technology Data Exchange (ETDEWEB)
Reilly, Nick; Wehrung, Michael; O' Dell, Ryan Andrew [Department of Physics and Astronomy, Bowling Green State University, Bowling Green, OH 43403 (United States); Sun, Liangfeng, E-mail: lsun@bgsu.edu [Department of Physics and Astronomy, Bowling Green State University, Bowling Green, OH 43403 (United States); Center for Photochemical Sciences, Bowling Green State University, Bowling Green, OH 43403 (United States)
2014-09-15
Ultrasmall colloidal lead sulfide quantum dots can increase the open circuit voltages of quantum-dot-based solar cells because of their large energy gap. Their small size and visible or near infrared light-emitting property make them attractive to the applications of biological fluorescence labeling. Through a modified organometallic route, we can synthesize lead sulfide quantum dots as small as 1.6 nm in diameter. The low reaction temperature and the addition of a chloroalkane cosolvent decrease the reaction rate, making it possible to obtain the ultrasmall quantum dots. - Highlights: • Ultrasmall colloidal PbS quantum dots as small as 1.6 nm in diameter are synthesized. • The quantum dots emit red light with photoluminescence peak at 760 nm. • The growth temperature is as low as 50 °C. • Addition of cosolvent 1,2-dichloroethane in the reaction decreases the reaction rate.
Energy Technology Data Exchange (ETDEWEB)
Mahato, Bipul Kumar; Rana, Bivas; Kumar, Dheeraj; Barman, Saswati; Barman, Anjan, E-mail: abarman@bose.res.in [Thematic Unit of Excellence on Nanodevice Technology, Department of Condensed Matter Physics and Material Sciences, S. N. Bose National Centre for Basic Sciences, Block JD, Sector III, Salt Lake, Kolkata 700098 (India); Sugimoto, Satoshi [Institute for Solid State Physics, University of Tokyo, 5-1-5 Kashiwanoha, Kashiwa, Chiba 277-8581 (Japan); Otani, YoshiChika [Institute for Solid State Physics, University of Tokyo, 5-1-5 Kashiwanoha, Kashiwa, Chiba 277-8581 (Japan); CEMS-RIKEN, 2-1 Hirosawa, Wako, Saitama 351-0198 (Japan)
2014-07-07
We demonstrate tunable spin wave spectrum in two-dimensional Ni{sub 80}Fe{sub 20} nanodot lattices by varying dot shape. A single collective mode in elliptical dot lattices transforms into three distinct modes for the half-elliptical, rectangular, and diamond dot lattices, albeit with different peak frequencies and intensities. A drastic change is observed for the triangular dots, where eight modes covering a broad band are observed. Using micromagnetic simulations, we characterized the modes as different localized, extended, and quantized modes, whose frequencies and spatial profiles are determined by a combination of internal field profiles within the nanodots and the stray magnetic field within the lattice.
Two-dimensional hole systems in indium-based quantum well heterostructures
Energy Technology Data Exchange (ETDEWEB)
Loher, Josef
2016-08-01
The complex spin-orbit interaction (SOI) of two-dimensional hole gas (2DHG) systems - the relativistic coupling of the hole spin degree of freedom to their movement in an electric field - is of fundamental interest in spin physics due to its key role for spin manipulation in spintronic devices. In this work, we were able to evaluate the tunability of Rashba-SOI-related parameters in the 2DHG system of InAlAs/InGaAs/InAs:Mn quantum well heterostructures experimentally by analyzing the hole density evolution of quantum interference effects at low magnetic fields. We achieved to cover a significant range of hole densities by the joint action of the variation of the manganese modulation doping concentration during molecular beam epitaxy and external field-effect-mediated manipulation of the 2D carrier density in Hall bar devices by a metallic topgate. Within these magnetotransport experiments, a reproducible phenomenon of remarkable robustness emerged in the transverse Hall magnetoresistivity of the indium 2DHG systems which are grown on a special InAlAs step-graded metamorphic buffer layer structure to compensate crystal lattice mismatch. As a consequence of the strain relaxation process, these material systems are characterized by anisotropic properties along different crystallographic directions. We identify a puzzling offset phenomenon in the zero-field Hall magnetoresistance and demonstrate it to be a universal effect in systems with spatially anisotropic transport properties.
Atomistic Analysis of Room Temperature Quantum Coherence in Two-Dimensional CdSe Nanostructures.
Pal, Sougata; Nijjar, Parmeet; Frauenheim, Thomas; Prezhdo, Oleg V
2017-03-02
Recent experiments on CdSe nanoplatelets synthesized with precisely controlled thickness that eliminates ensemble disorder have allowed accurate measurement of quantum coherence at room temperature. Matching exactly the CdSe cores of the experimentally studied particles and considering several defects, we establish the atomistic origins of the loss of coherence between heavy and light hole excitations in two-dimensional CdSe and CdSe/CdZnS core/shell structures. The coherence times obtained using molecular dynamics based on tight-binding density functional theory are in excellent agreement with the measured values. We show that a long coherence time is a consequence of both small fluctuations in the energy gap between the excited state pair, which is much less than thermal energy, and a slow decay of correlation between the energies of the two states. Anionic defects at the core/shell interface have little effect on the coherence lifetime, while cationic defects strongly perturb the electronic structure, destroying the experimentally observed coherence. By coupling to the same phonon modes, the heavy and light holes synchronize their energy fluctuations, facilitating long-lived coherence. We further demonstrate that the electronic excitations are localized close to the surface of these narrow nanoscale systems, and therefore, they couple most strongly to surface acoustic phonons. The established features of electron-phonon coupling and the influence of defects, surfaces, and core/shell interfaces provide important insights into quantum coherence in nanoscale materials in general.
Excited states of two-dimensional hydrogen atom in tilted magnetic field: Quantum chaos
Koval, Eugene A.; Koval, Oksana A.
2017-09-01
The aim of the current work is the research of the influence of a tilted magnetic field direction on the spectrum and the energy level spacing distribution of a two-dimensional (2D) hydrogen atom and of an exciton in GaAs/Al0.33Ga0.67As quantum well. It was discovered that the quantum chaos (QC) is initiated with an increasing angle α between the magnetic field direction and the normal to the atomic plane. It is characterized by the repulsion of levels leading to the eliminating of the shell structure and by changing the spectrum statistical properties. The statement about the initiation of chaos and its dominance over regular motion with increasing angle α is confirmed by the results of our calculations of the classical dynamics presented in this paper. The evolution of the spatial distribution of the square of the absolute value of the wave function at an increasing angle α was observed. The differences of calculated dependencies of energies for various excited states on the tilt angle at a wide range of the magnetic field strength were described.
Polarized heat current generated by quantum pumping in two-dimensional topological insulators
Ronetti, F.; Carrega, M.; Ferraro, D.; Rech, J.; Jonckheere, T.; Martin, T.; Sassetti, M.
2017-03-01
We consider the transport properties of a two-dimensional topological insulator in a double quantum point contact geometry in the presence of a time-dependent external field. In the proposed setup an external gate is placed above a single constriction and it couples only with electrons belonging to the top edge. This asymmetric configuration and the presence of an ac signal allow for a quantum pumping mechanism, which, in turn, can generate finite heat and charge currents in an unbiased device configuration. A microscopic model for coupling with the external time-dependent gate potential is developed and the induced finite heat and charge currents are investigated. We demonstrate that in the noninteracting case, heat flow is associated with a single spin component, due to the helical nature of the edge states, and therefore a finite and polarized heat current is obtained in this configuration. The presence of e -e interchannel interactions strongly affects the current signal, lowering the degree of polarization of the system. Finally, we also show that separate heat and charge flows can be achieved, varying the amplitude of the external gate.
Czarnik, Piotr; Dziarmaga, Jacek; Oleś, Andrzej M.
2016-05-01
Progress in describing thermodynamic phase transitions in quantum systems is obtained by noticing that the Gibbs operator e-β H for a two-dimensional (2D) lattice system with a Hamiltonian H can be represented by a three-dimensional tensor network, the third dimension being the imaginary time (inverse temperature) β . Coarse graining the network along β results in a 2D projected entangled-pair operator (PEPO) with a finite bond dimension D . The coarse graining is performed by a tree tensor network of isometries. The isometries are optimized variationally, taking into account full tensor environment, to maximize the accuracy of the PEPO. The algorithm is applied to the isotropic quantum compass model on an infinite square lattice near a symmetry-breaking phase transition at finite temperature. From the linear susceptibility in the symmetric phase and the order parameter in the symmetry-broken phase, the critical temperature is estimated at Tc=0.0606 (4 ) J , where J is the isotropic coupling constant between S =1/2 pseudospins.
POLARON IN CYLINDRICAL AND SPHERICAL QUANTUM DOTS
Directory of Open Access Journals (Sweden)
L.C.Fai
2004-01-01
Full Text Available Polaron states in cylindrical and spherical quantum dots with parabolic confinement potentials are investigated applying the Feynman variational principle. It is observed that for both kinds of quantum dots the polaron energy and mass increase with the increase of Frohlich electron-phonon coupling constant and confinement frequency. In the case of a spherical quantum dot, the polaron energy for the strong coupling is found to be greater than that of a cylindrical quantum dot. The energy and mass are found to be monotonically increasing functions of the coupling constant and the confinement frequency.
Activation of silicon quantum dots for emission
Institute of Scientific and Technical Information of China (English)
Huang Wei-Qi; Miao Xin-Jian; Huang Zhong-Mei; Liu Shi-Rong; Qin Chao-Jian
2012-01-01
The emission of silicon quantum dots is weak when their surface is passivated well. Oxygen or nitrogen on the surface of silicon quantum dots can break the passivation to form localized electronic states in the band gap to generate active centers where stronger emission occurs.From this point of view,we can build up radiative matter for emission.Emissions of various wavelengths can be obtained by controlling the surface bonds of silicon quantum dots.Our experimental results demonstrate that annealing is important in the treatment of the activation,and stimulated emissions at about 600 and 700 nm take place on active silicon quantum dots.
Synthetic Developments of Nontoxic Quantum Dots.
Das, Adita; Snee, Preston T
2016-03-03
Semiconductor nanocrystals, or quantum dots (QDs), are candidates for biological sensing, photovoltaics, and catalysis due to their unique photophysical properties. The most studied QDs are composed of heavy metals like cadmium and lead. However, this engenders concerns over heavy metal toxicity. To address this issue, numerous studies have explored the development of nontoxic (or more accurately less toxic) quantum dots. In this Review, we select three major classes of nontoxic quantum dots composed of carbon, silicon and Group I-III-VI elements and discuss the myriad of synthetic strategies and surface modification methods to synthesize quantum dots composed of these material systems.
Nanostructure assembly of indium sulphide quantum dots and their characterization.
Vigneashwari, B; Ravichandran, V; Parameswaran, P; Dash, S; Tyagi, A K
2008-02-01
Nanocrystals (approximately 5 nm) of the semiconducting wide band gap material beta-In2S3 obtained by chemical synthesis through a hydrothermal route were characterized for phase and compositional purity. These nanoparticles exhibited quantum confinement characteristics as revealed by a blue-shifted optical absorption. These quantum dots of beta-In2S3 were electrically driven from a monodisperse colloidal suspension on to conducting glass substrates by Electophoretic Deposition (EPD) technique and nanostructural thin films were obtained. The crystalline and morphological structures of these deposits were investigated by X-ray diffraction and nanoscopic techniques. We report here that certain interesting nanostructural morphologies were observed in the two-dimensional quantum dot assemblies of beta-In2S3. The effect of the controlling parameters on the cluster growth and deposit integrity was also systematically studied through a series of experiments and the results are reported here.
Spin transport through quantum dots
Energy Technology Data Exchange (ETDEWEB)
Lima, A.T. da Cunha; Anda, Enrique V. [Pontificia Univ. Catolica do Rio de Janeiro (PUC-Rio), RJ (Brazil)
2003-07-01
Full text: We investigate the spin polarized transport properties of a nanoscopic device constituted by a quantum dot connected to two leads. The electrical current circulates with a spin polarization that is modulated via a gate potential that controls the intensity of the spin-orbit coupling, the Rashba effect. We study a polarized field-effect transistor when one of its parts is constituted by a small quantum dot, which energies are controlled by another gate potential operating inside the confined region. The high confinement and correlation suffered by the charges inside the dot gives rise to novel phenomena. We show that through the manipulation of the gate potential applied to the dot it is possible to control, in a very efficient way, the intensity and polarization of the current that goes along the system. Other crucial parameters to be varied in order to understand the behavior of this system are the intensity of the external applied electric and magnetic field. The system is represented by the Anderson Impurity Hamiltonian summed to a spin-orbit interaction, which describes the Rashba effect. To obtain the current of this out-of-equilibrium system we use the Keldysh formalism.The solution of the Green function are compatible with the Coulomb blockade regime. We show that under the effect of a external magnetic field, if the dot is small enough the device operates as a complete spin filter that can be controlled by the gate potential. The behavior of this device when it is injected into it a polarized current and modulated by the Rashba effect is as well studied. (author)
Quantum optics with quantum dots in photonic nanowires
DEFF Research Database (Denmark)
We will review recent studies performed on InAs quantum dots embedded in GaAs photonic wires, which highlight the strong interest of the photonic wire geometry for quantum optics experiments and quantum optoelectronic devices.......We will review recent studies performed on InAs quantum dots embedded in GaAs photonic wires, which highlight the strong interest of the photonic wire geometry for quantum optics experiments and quantum optoelectronic devices....
Quantum Optics with Quantum Dots in Photonic Nanowires
DEFF Research Database (Denmark)
Gérard, J.-M.; Claudon, J.; Bleuse, J.;
2011-01-01
We review recent studies performed on InAs quantum dots embedded in GaAs photonic wires, which highlight the strong interest of the photonic wire geometry for quantum optics experiments and quantum optoelectronic devices.......We review recent studies performed on InAs quantum dots embedded in GaAs photonic wires, which highlight the strong interest of the photonic wire geometry for quantum optics experiments and quantum optoelectronic devices....
Colloidal quantum dots as optoelectronic elements
Vasudev, Milana; Yamanaka, Takayuki; Sun, Ke; Li, Yang; Yang, Jianyong; Ramadurai, Dinakar; Stroscio, Michael A.; Dutta, Mitra
2007-02-01
Novel optoelectronic systems based on ensembles of semiconductor nanocrystals are addressed in this paper. Colloidal semiconductor quantum dots and related quantum-wire structures have been characterized optically; these optical measurements include those made on self-assembled monolayers of DNA molecules terminated on one end with a common substrate and on the other end with TiO II quantum dots. The electronic properties of these structures are modeled and compared with experiment. The characterization and application of ensembles of colloidal quantum dots with molecular interconnects are considered. The chemically-directed assembly of ensembles of colloidal quantum dots with biomolecular interconnects is demonstrated with quantum dot densities in excess of 10 +17 cm -3. A number of novel photodetectors have been designed based on the combined use of double-barrier quantum-well injectors, colloidal quantum dots, and conductive polymers. Optoelectronic devices including photodetectors and solar cells based on threedimensional ensembles of quantum dots are considered along with underlying phenomena such as miniband formation and the robustness of minibands to displacements of quantum dots in the ensemble.
Chiral quantum dot based materials
Govan, Joseph; Loudon, Alexander; Baranov, Alexander V.; Fedorov, Anatoly V.; Gun'ko, Yurii
2014-05-01
Recently, the use of stereospecific chiral stabilising molecules has also opened another avenue of interest in the area of quantum dot (QD) research. The main goal of our research is to develop new types of technologically important quantum dot materials containing chiral defects, study their properties and explore their applications. The utilisation of chiral penicillamine stabilisers allowed the preparation of new water soluble white emitting CdS quantum nanostructures which demonstrated circular dichroism in the band-edge region of the spectrum. It was also demonstrated that all three types of QDs (D-, L-, and Rac penicillamine stabilised) show very broad emission bands between 400 and 700 nm due to defects or trap states on the surfaces of the nanocrystals. In this work the chiral CdS based quantum nanostructures have also been doped by copper metal ions and new chiral penicilamine stabilized CuS nanoparticles have been prepared and investigated. It was found that copper doping had a strong effect at low levels in the synthesis of chiral CdS nanostructures. We expect that this research will open new horizons in the chemistry of chiral nanomaterials and their application in biotechnology, sensing and asymmetric synthesis.
Institute of Scientific and Technical Information of China (English)
李秀平; 阎维贤
2004-01-01
We investigate the evolution behaviour of electron-hole pair wavepacket in optically excited square quantum-dot arrays driven by in-plane (x-y plane) uniform electric field E (viz, E ＝ Exex + Eyey, ex,ey are unit vectors along x and y directions respectively), in the time domain. It is found that if the ratio of the x-component electric field Ex to the y-component electric field Ey is a rational p/q (p and q being coprime integer numbers),the wavepackets undergo a time-periodic breathing mode, with the period 2πp/ωBx, where ωBx ＝ eExa/h, with a being the lattice constant of square dot arrays, h being Planck's constant, e being the electron charge. This finding provides a time-domain demonstration of the recent spectral result [Phys. Rev. Lett. 86 (2001)3116].
Tunable two-dimensional arrays of single Rydberg atoms for realizing quantum Ising models.
Labuhn, Henning; Barredo, Daniel; Ravets, Sylvain; de Léséleuc, Sylvain; Macrì, Tommaso; Lahaye, Thierry; Browaeys, Antoine
2016-06-30
Spin models are the prime example of simplified many-body Hamiltonians used to model complex, strongly correlated real-world materials. However, despite the simplified character of such models, their dynamics often cannot be simulated exactly on classical computers when the number of particles exceeds a few tens. For this reason, quantum simulation of spin Hamiltonians using the tools of atomic and molecular physics has become a very active field over the past years, using ultracold atoms or molecules in optical lattices, or trapped ions. All of these approaches have their own strengths and limitations. Here we report an alternative platform for the study of spin systems, using individual atoms trapped in tunable two-dimensional arrays of optical microtraps with arbitrary geometries, where filling fractions range from 60 to 100 per cent. When excited to high-energy Rydberg D states, the atoms undergo strong interactions whose anisotropic character opens the way to simulating exotic matter. We illustrate the versatility of our system by studying the dynamics of a quantum Ising-like spin-1/2 system in a transverse field with up to 30 spins, for a variety of geometries in one and two dimensions, and for a wide range of interaction strengths. For geometries where the anisotropy is expected to have small effects on the dynamics, we find excellent agreement with ab initio simulations of the spin-1/2 system, while for strongly anisotropic situations the multilevel structure of the D states has a measurable influence. Our findings establish arrays of single Rydberg atoms as a versatile platform for the study of quantum magnetism.
Quantum Dot Spectrum Converters for Enhanced High Efficiency Photovoltaics Project
National Aeronautics and Space Administration — This research proposes to enhance solar cell efficiency, radiation resistance and affordability. The Quantum Dot Spectrum Converter (QDSC) disperses quantum dots...
Exciton in type-II quantum dot
Energy Technology Data Exchange (ETDEWEB)
Sierra-Ortega, J; Escorcia, R A [Universidad del Magdalena, A. A. 731, Santa Marta (Colombia); Mikhailov, I D, E-mail: jsierraortega@gmail.co [Universidad Industrial de Santander, A. A. 678, Bucaramanga (Colombia)
2009-05-01
We study the quantum-size effect and the influence of the external magnetic field on the exciton ground state energy in the type-II InP quantum disk, lens and pyramid deposited on a wetting layer and embedded in a GaInP matrix. We show that the charge distribution over and below quantum dot and wetting layer induced by trapped exciton strongly depends on the quantum dot morphology and the strength of the magnetic field.
Colloidal quantum dot photodetectors
Konstantatos, Gerasimos
2011-05-01
We review recent progress in light sensors based on solution-processed materials. Spin-coated semiconductors can readily be integrated with many substrates including as a post-process atop CMOS silicon and flexible electronics. We focus in particular on visible-, near-infrared, and short-wavelength infrared photodetectors based on size-effect-tuned semiconductor nanoparticles made using quantum-confined PbS, PbSe, Bi 2S3, and In2S3. These devices have in recent years achieved room-temperature D values above 1013 Jones, while fully-depleted photodiodes based on these same materials have achieved MHz response combined with 1012 Jones sensitivities. We discuss the nanoparticle synthesis, the materials processing, integrability, temperature stability, physical operation, and applied performance of this class of devices. © 2010 Elsevier Ltd. All rights reserved.
Quantum control study of ultrafast optical responses in semiconductor quantum dot devices.
Huang, Jung Y; Lin, Chien Y; Liu, Wei-Sheng; Chyi, Jen-Inn
2014-12-15
Two quantum control spectroscopic techniques were applied to study InAs quantum dot (QD) devices, which contain different strain-reducing layers. By adaptively control light matter interaction, a delayed resonant response from the InAs QDs was found to be encoded into the optimal phase profile of ultrafast optical pulse used. We verified the delayed resonant response to originate from excitons coupled to acoustic phonons of InAs QDs with two-dimensional coherent spectroscopy. Our study yields valuable dynamical information that can deepen our understanding of the coherent coupling process of exciton in the quantum-confined systems.
Experimental study of two-dimensional quantum Wigner solid in zero magnetic field
Energy Technology Data Exchange (ETDEWEB)
Huang, Jian [Department of Physics and Astronomy, Wayne State University, Detroit, MI 48201 (United States); Pfeiffer, L. N.; West, K. W. [Department of Electrical Engineering, Princeton University, Princeton, NJ 08544 (United States)
2014-03-31
At temperatures T → 0, strongly interacting two-dimensional (2D) electron systems manifest characteristic insulating behaviors that are key for understanding the nature of the ground state in light of the interplay between disorder and electron-electron interaction. In contrast to the hopping conductance demonstrated in the insulating side of the metal-to-insulator transition, the ultra-high quality 2D systems exhibit nonactivated T-dependence of the conductivity even for dilute carrier concentrations down to 7×10{sup 8} cm{sup −2}. The apparent metal-to-insulator transition (MIT) occurs for a large r{sub s} value around 40 for which a Wigner Crystalllization is expected. The magnetoresistance for a series of carrier densities in the vicinity of the transition exhibits a characteristic sign change in weak perpendicular magnetic field. Within the Wigner Crystallization regime (with r{sub s} > 40), we report an experimental observation of a characteristic nonlinear threshold behavior from a high-resolution dc dynamical response as an evidence for aWigner crystallization in high-purity GaAs 2D hole systems in zero magnetic field. The system under an increasing current drive exhibits voltage oscillations with negative differential resistance. They confirm the coexistence of a moving crystal along with striped edge states as observed for electrons on helium surfaces. Moreover, the threshold is well below the typical classical levels due to a different pinning and depinning mechanism that is possibly related to quantum processes.
Experimental study of two-dimensional quantum Wigner solid in zero magnetic field
Huang, Jian; Pfeiffer, L. N.; West, K. W.
2014-03-01
At temperatures T → 0, strongly interacting two-dimensional (2D) electron systems manifest characteristic insulating behaviors that are key for understanding the nature of the ground state in light of the interplay between disorder and electron-electron interaction. In contrast to the hopping conductance demonstrated in the insulating side of the metal-to-insulator transition, the ultra-high quality 2D systems exhibit nonactivated T-dependence of the conductivity even for dilute carrier concentrations down to 7×108 cm-2. The apparent metal-to-insulator transition (MIT) occurs for a large rs value around 40 for which a Wigner Crystalllization is expected. The magnetoresistance for a series of carrier densities in the vicinity of the transition exhibits a characteristic sign change in weak perpendicular magnetic field. Within the Wigner Crystallization regime (with rs > 40), we report an experimental observation of a characteristic nonlinear threshold behavior from a high-resolution dc dynamical response as an evidence for aWigner crystallization in high-purity GaAs 2D hole systems in zero magnetic field. The system under an increasing current drive exhibits voltage oscillations with negative differential resistance. They confirm the coexistence of a moving crystal along with striped edge states as observed for electrons on helium surfaces. Moreover, the threshold is well below the typical classical levels due to a different pinning and depinning mechanism that is possibly related to quantum processes.
Zhou, Jian; Jena, Puru
2017-02-01
While most of the two-dimensional (2D) topological crystalline insulators (TCIs) belong to group IV-VI narrow-band-gap semiconductors in a square lattice, in the present work we predict a TCI family based on transition metal intercalated compounds in a hexagonal lattice. First-principles calculations combined with a substrate-fixed globally optimal structural search technique show that a layer of Os prefers a uniform distribution between two graphene sheets. Band dispersion calculations reveal a Dirac point and a Dirac nodal ring near the Fermi level. The Dirac point is ascribed to the hybridization of e2 and e2* orbitals, and the Dirac ring is formed due to dispersion of s and e1* orbitals. Upon inclusion of spin-orbit coupling, these Dirac states open topologically nontrivial local band gaps, which are characterized by nonzero mirror Chern numbers. The quantum spin Hall effect is also observed by integrating the spin Berry curvature in the Brillouin zone. In contrast to the 2D group IV-VI TCIs whose band inversions at X and Y points are "locked" by C4 rotation symmetry, here the relative energy of two local band gaps can be manipulated by in-plane biaxial strains. Some other similar intercalation compounds are also shown to be topologically nontrivial. Our work extends the 2D TCI family into a hexagonal lattice composed of transition metals.
Topological Phase and Half-Integer Orbital Angular Momenta in Circular Quantum Dots
Kuleshov, V. M.; Mur, V. D.; Narozhny, N. B.; Lozovik, Yu. E.
2016-12-01
We show that there exists a non-trivial topological phase in circular two-dimensional quantum dots with an odd number of electrons. The possible non-zero value of this phase is explained by axial symmetry of two-dimensional quantum systems. The particular value of this phase (π ) is fixed by T-invariance and the Pauli exclusion principle and leads to half-integer values of the angular orbital momentum for ground states of such systems. This conclusion agrees with the experimental data for ground-state energies of few-electron circular quantum dots in perpendicular magnetic field (Schmidt et al. in Phys Rev B 51:5570, 1995). Hence, these data may be considered as the first experimental evidence for the existence of topological phase leading to half-integer quantization of the orbital angular momentum in circular quantum dots with an odd number of electrons.
Optical studies of capped quantum dots
Wuister, S.F.
2005-01-01
This thesis describes the synthesis and spectroscopy of CdSe and CdTe semiconductor quantum dots (QDs). The first chapter gives an introduction into the unique size dependent properties of semiconductor quantum dots. Highly luminescent QDs of CdSe and CdTe were prepared via a high temperature method
Detecting the chirality for coupled quantum dots
Energy Technology Data Exchange (ETDEWEB)
Cao Huijuan [Institute for Condensed Matter Physics, School of Physics and Telecommunication Engineering, South China Normal University, Guangzhou 510631 (China); Hu Lian [Institute for Condensed Matter Physics, School of Physics and Telecommunication Engineering, South China Normal University, Guangzhou 510631 (China)], E-mail: huliancaohj@yahoo.com
2008-04-21
We propose a scheme to detect the chirality for a system consisting of three coupled quantum dots. The chirality is found to be determined by the frequency of the transition between chiral states under the chiral symmetry broken perturbation. The results are important to construct quantum gates and to demonstrate chiral entangle states in the triangle spin dots.
Optically active quantum-dot molecules.
Shlykov, Alexander I; Baimuratov, Anvar S; Baranov, Alexander V; Fedorov, Anatoly V; Rukhlenko, Ivan D
2017-02-20
Chiral molecules made of coupled achiral semiconductor nanocrystals, also known as quantum dots, show great promise for photonic applications owing to their prospective uses as configurable building blocks for optically active structures, materials, and devices. Here we present a simple model of optically active quantum-dot molecules, in which each of the quantum dots is assigned a dipole moment associated with the fundamental interband transition between the size-quantized states of its confined charge carriers. This model is used to analytically calculate the rotatory strengths of optical transitions occurring upon the excitation of chiral dimers, trimers, and tetramers of general configurations. The rotatory strengths of such quantum-dot molecules are found to exceed the typical rotatory strengths of chiral molecules by five to six orders of magnitude. We also study how the optical activity of quantum-dot molecules shows up in their circular dichroism spectra when the energy gap between the molecular states is much smaller than the states' lifetime, and maximize the strengths of the circular dichroism peaks by optimizing orientations of the quantum dots in the molecules. Our analytical results provide clear design guidelines for quantum-dot molecules and can prove useful in engineering optically active quantum-dot supercrystals and photonic devices.
Research on Self-Assembling Quantum Dots.
1995-10-30
0K. in a second phase of this contract we turned our efforts to the fabrication and studies of self assembled quantum dots . We first demonstrated a...method for producing InAs-GasAs self assembled quantum dots (SAD) using MBE. (AN)
Thick-shell nanocrystal quantum dots
Hollingsworth, Jennifer A.; Chen, Yongfen; Klimov, Victor I.; Htoon, Han; Vela, Javier
2011-05-03
Colloidal nanocrystal quantum dots comprising an inner core having an average diameter of at least 1.5 nm and an outer shell, where said outer shell comprises multiple monolayers, wherein at least 30% of the quantum dots have an on-time fraction of 0.80 or greater under continuous excitation conditions for a period of time of at least 10 minutes.
Optical Properties of Semiconductor Quantum Dots
Perinetti, U.
2011-01-01
This thesis presents different optical experiments performed on semiconductor quantum dots. These structures allow to confine a small number of electrons and holes to a tiny region of space, some nm across. The aim of this work was to study the basic properties of different types of quantum dots
Optical Properties of Semiconductor Quantum Dots
Perinetti, U.
2011-01-01
This thesis presents different optical experiments performed on semiconductor quantum dots. These structures allow to confine a small number of electrons and holes to a tiny region of space, some nm across. The aim of this work was to study the basic properties of different types of quantum dots mad
Ground State of a Two-Electron Quantum Dot with a Gaussian Confining Potential
Institute of Scientific and Technical Information of China (English)
XIE Wen-Fang
2006-01-01
We investigate the ground-state properties of a two-dimensional two-electron quantum dot with a Gaussian confining potential under the influence of perpendicular homogeneous magnetic field. Calculations are carried out by using the method of numerical diagonalization of Hamiltonian matrix within the effective-mass approximation. A ground-state behaviour (singlet→triplet state transitions) as a function of the strength of a magnetic field has been found. It is found that the dot radius R of the Gaussian potential is important for the ground-state transition and the feature of ground-state for the Gaussian potential quantum dot (QD), and the parabolic potential QDs are similar when R is larger. The larger the quantum dot radius, the smaller the magnetic field for the singlet-triplet transition of the ground-state of two interacting electrons in the Gaussian quantum dot.
An, Taeyang; Cha, Min-Chul
2013-03-01
We study the superfluid-insulator quantum phase transition in a disordered two-dimensional quantum rotor model with random on-site interactions in the presence of particle-hole symmetry. Via worm-algorithm Monte Carlo calculations of superfluid density and compressibility, we find the dynamical critical exponent z ~ 1 . 13 (2) and the correlation length critical exponent 1 / ν ~ 1 . 1 (1) . These exponents suggest that the insulating phase is a incompressible Mott glass rather than a Bose glass.
Biocompatible quantum dots for biological applications.
Rosenthal, Sandra J; Chang, Jerry C; Kovtun, Oleg; McBride, James R; Tomlinson, Ian D
2011-01-28
Semiconductor quantum dots are quickly becoming a critical diagnostic tool for discerning cellular function at the molecular level. Their high brightness, long-lasting, size-tunable, and narrow luminescence set them apart from conventional fluorescence dyes. Quantum dots are being developed for a variety of biologically oriented applications, including fluorescent assays for drug discovery, disease detection, single protein tracking, and intracellular reporting. This review introduces the science behind quantum dots and describes how they are made biologically compatible. Several applications are also included, illustrating strategies toward target specificity, and are followed by a discussion on the limitations of quantum dot approaches. The article is concluded with a look at the future direction of quantum dots.
Realization of electrically tunable single quantum dot nanocavities
Energy Technology Data Exchange (ETDEWEB)
Hofbauer, Felix Florian Georg
2009-03-15
We investigated the design, fabrication and optical investigation of electrically tunable single quantum dot-photonic crystal defect nanocavities operating in both the weak and strong coupling regimes of the light matter interaction. We demonstrate that the quantum confined Stark effect can be employed to quickly and reversibly switch the dot-cavity coupling, simply by varying a gate voltage. Our results show that exciton transitions from individual dots can be tuned by up to {proportional_to}4 meV relative to the nanocavity mode, before the emission quenches due to carrier tunneling escape from the dots. We directly probe spontaneous emission, irreversible polariton decay and the statistics of the emitted photons from a single-dot nanocavity in the weak and strong coupling regimes. New information is obtained on the nature of the dot-cavity coupling in the weak coupling regime and electrical control of zero dimensional polaritons is demonstrated for the first time. The structures investigated are p-i-n photodiodes consisting of an 180nm thick free-standing GaAs membrane into which a two dimensional photonic crystal is formed by etching a triangular lattice of air holes. Low mode volume nanocavities (V{sub mode}<1.6 ({lambda}/n){sup 3}) are realized by omitting 3 holes in a line to form L3 cavities and a single layer of InGaAs self-assembled quantum dots is embedded into the midpoint of the membrane. The nanocavities are electrically contacted via 35 nm thick p- and n-doped contact layers in the GaAs membrane. In the weak coupling regime, time resolved spectroscopy reveals a {proportional_to}7 x shortening of the spontaneous emission lifetime as the dot is tuned through the nanocavity mode, due to the Purcell effect. Upon strongly detuning the same quantum dot transition from the nanocavity mode we observe an additional {proportional_to}8 x lengthening of the spontaneous emission lifetime. These observations unequivocally highlight two regimes of dot
Facile synthesis and photoluminescence mechanism of graphene quantum dots
Energy Technology Data Exchange (ETDEWEB)
Yang, Ping; Zhou, Ligang; Zhang, Shenli; Pan, Wei, E-mail: sjtushelwill@sjtu.edu.cn; Shen, Wenzhong, E-mail: wzshen@sjtu.edu.cn [Laboratory of Condensed Matter Spectroscopy and Opto-Electronic Physics, and Key Laboratory of Artificial Structures and Quantum Control (Ministry of Education), Department of Physics and Astronomy, Shanghai Jiao Tong University, Shanghai 200240 (China); Wan, Neng [SEU-FEI Nano Pico Center, Key Laboratory of MEMS of Ministry of Education, School of Electronics Science and Engineering, Southeast University, Nanjing 210096 (China)
2014-12-28
We report a facile hydrothermal synthesis of intrinsic fluorescent graphene quantum dots (GQDs) with two-dimensional morphology. This synthesis uses glucose, concentrate sulfuric acid, and deionized water as reagents. Concentrated sulfuric acid is found to play a key role in controlling the transformation of as-prepared hydrothermal products from amorphous carbon nanodots to well-crystallized GQDs. These GQDs show typical absorption characteristic for graphene, and have nearly excitation-independent ultraviolet and blue intrinsic emissions. Temperature-dependent PL measurements have demonstrated strong electron-electron scattering and electron-phonon interactions, suggesting a similar temperature behavior of GQDs to inorganic semiconductor quantum dots. According to optical studies, the ultraviolet emission is found to originate from the recombination of electron-hole pairs localized in the C=C bonds, while the blue emission is from the electron transition of sp{sup 2} domains.
Phonons in Ge/Si superlattices with Ge quantum dots
Milekhin, A G; Pchelyakov, O P; Schulze, S; Zahn, D R T
2001-01-01
Ge/Si superlattices with Ge quantum dots obtained by means of molecular-beam epitaxy were investigated by means of light Raman scattering under resonance conditions. These structures are shown to have oscillation properties of both two-dimensional and zero-dimensional objects. Within spectrum low-frequency range one observes twisted acoustic phonons (up to 15 order) typical for planar superlattices. Lines of acoustic phonons are overlapped with a wide band of continuous emission. Analysis of frequencies of Ge and Ge-Si optical phonons shows that Ge quantum dots are pseudoamorphous ones and mixing of Ge and Si atoms is a negligible one. One detected low-frequency shift of longitudinal optical phonons at laser excitation energy increase (2.54-2.71 eV)
Tailoring Magnetism in Quantum Dots
Zutic, Igor; Abolfath, Ramin; Hawrylak, Pawel
2007-03-01
We study magnetism in magnetically doped quantum dots as a function of particle numbers, temperature, confining potential, and the strength of Coulomb interaction screening. We show that magnetism can be tailored by controlling the electron-electron Coulomb interaction, even without changing the number of particles. The interplay of strong Coulomb interactions and quantum confinement leads to enhanced inhomogeneous magnetization which persists at substantially higher temperatures than in the non-interacting case or in the bulk-like dilute magnetic semiconductors. We predict a series of electronic spin transitions which arise from the competition between the many-body gap and magnetic thermal fluctuations. Cond-mat/0612489. [1] R. Abolfath, P. Hawrylak, I. Zuti'c, preprint.
Iwaki, Sunao; Bonmassar, Giorgio; Belliveau, John W
2013-09-01
Recent neuroimaging studies implicate that both the dorsal and ventral visual pathways, as well as the middle temporal (MT) areas which are critical for the perception of visual motion, are involved in the perception of three-dimensional (3D) structure from two-dimensional (2D) motion (3D-SFM). However, the neural dynamics underlying the reconstruction of a 3D object from 2D optic flow is not known. Here we combined magnetoencephalography (MEG) and functional MRI (fMRI) measurements to investigate the spatiotemporal brain dynamics during 3D-SFM. We manipulated parametrically the coherence of randomly moving groups of dots to create different levels of 3D perception and to study the associated changes in brain activity. At different latencies, the posterior infero-temporal (pIT), the parieto-occipital (PO), and the intraparietal (IP) regions showed increased neural activity during highly coherent motion conditions in which subjects perceived a robust 3D object. Causality analysis between these regions indicated significant causal influence from IP to pIT and from pIT to PO only in conditions where subjects perceived a robust 3D object. Current results suggest that the perception of a 3D object from 2D motion includes integration of global motion and 3D mental image processing, as well as object recognition that are accomplished by interactions between the dorsal and ventral visual pathways.
Coherent optoelectronics with single quantum dots
Energy Technology Data Exchange (ETDEWEB)
Zrenner, A; Ester, P; Michaelis de Vasconcellos, S; Huebner, M C; Lackmann, L; Stufler, S [Universitaet Paderborn, Department Physik, Warburger Strasse 100, D-33098 Paderborn (Germany); Bichler, M [Walter Schottky Institut, Technische Universitaet Muenchen, Am Coulombwall, D-85748 Garching (Germany)], E-mail: zrenner@mail.upb.de
2008-11-12
The optical properties of semiconductor quantum dots are in many respects similar to those of atoms. Since quantum dots can be defined by state-of-the-art semiconductor technologies, they exhibit long-term stability and allow for well-controlled and efficient interactions with both optical and electrical fields. Resonant ps excitation of single quantum dot photodiodes leads to new classes of coherent optoelectronic functions and devices, which exhibit precise state preparation, phase-sensitive optical manipulations and the control of quantum states by electrical fields.
Coherent optoelectronics with single quantum dots
Zrenner, A.; Ester, P.; Michaelis de Vasconcellos, S.; Hübner, M. C.; Lackmann, L.; Stufler, S.; Bichler, M.
2008-11-01
The optical properties of semiconductor quantum dots are in many respects similar to those of atoms. Since quantum dots can be defined by state-of-the-art semiconductor technologies, they exhibit long-term stability and allow for well-controlled and efficient interactions with both optical and electrical fields. Resonant ps excitation of single quantum dot photodiodes leads to new classes of coherent optoelectronic functions and devices, which exhibit precise state preparation, phase-sensitive optical manipulations and the control of quantum states by electrical fields.
Quantum dot devices for optical communications
DEFF Research Database (Denmark)
Mørk, Jesper
2005-01-01
. The main property of semiconductor quantum dots compared to bulk material or even quantum well structures is the discrete nature of the allowed states, which means that inversion of the medium can be obtained for very low electron densities. This has led to the fabrication of quantum dot lasers with record......-low threshold currents and amplifiers with record-high power levels. In this tutorial we will review the basic properties of quantum dots, emphasizing the properties which are important for laser and amplifier applications, as well as devices for all-optical signal processing. The high-speed properties...
Electron transport in quantum dots
2003-01-01
When I was contacted by Kluwer Academic Publishers in the Fall of 200 I, inviting me to edit a volume of papers on the issue of electron transport in quantum dots, I was excited by what I saw as an ideal opportunity to provide an overview of a field of research that has made significant contributions in recent years, both to our understanding of fundamental physics, and to the development of novel nanoelectronic technologies. The need for such a volume seemed to be made more pressing by the fact that few comprehensive reviews of this topic have appeared in the literature, in spite of the vast activity in this area over the course of the last decade or so. With this motivation, I set out to try to compile a volume that would fairly reflect the wide range of opinions that has emerged in the study of electron transport in quantum dots. Indeed, there has been no effort on my part to ensure any consistency between the different chapters, since I would prefer that this volume instead serve as a useful forum for the...
Spin transport in the two-dimensional quantum disordered anisotropic Heisenberg model
Energy Technology Data Exchange (ETDEWEB)
Lima, L.S. [Departamento de Física e Matemática, Centro Federal de Educação Tecnológica de Minas Gerais, 30510-000 Belo Horizonte, MG (Brazil); Pires, A.S.T.; Costa, B.V. [Departamento de Física ICEx, UFMG, CP 702, 31270-901 Belo Horizonte, MG (Brazil)
2014-12-15
We use the self consistent harmonic approximation together with the Linear Response Theory to study the effect of nonmagnetic disorder on spin transport in the quantum diluted two-dimensional anisotropic Heisenberg model with spin S=1 in a square lattice. The model has a BKT transition at zero dilution. We calculate the regular part of the spin conductivity σ{sup reg}(ω) and the Drude weight D{sub S}(T) as a function of the non-magnetic concentration, x. Our calculations show that the spin conductivity drops abruptly to zero at x{sub c}{sup SCHA}≈0.5 indicating that the system changes from an ideal spin conductor state to an insulator. This value is far above the site percolation threshold x{sub c}{sup site}≈0.41. Although the SCHA fails in determining precisely the percolation threshold, both the spin conductivity and the Drude weight show a quite regular behavior inside 0≤x≤x{sub c}{sup SCHA} indicating that the transition stays in the same universality class all along the interval. - Highlights: • The site dilution generates a large influence on regular part of the spin conductivity, σ{sup reg}(ω), and in the Drude weight, D(T). • In a concentration of impurities about x≈0.5, the regular part of the spin conductivity and the Drude weight fall to zero. • In this point we have a change in the state of the system from an ideal spin conductor to a spin insulator.
Kwac, Kijeong; Lee, Chewook; Jung, Yousung; Han, Jaebeom; Kwak, Kyungwon; Zheng, Junrong; Fayer, M D; Cho, Minhaeng
2006-12-28
Molecular dynamics (MD) simulations and quantum mechanical electronic structure calculations are used to investigate the nature and dynamics of the phenol-benzene complex in the mixed solvent, benzene/CCl4. Under thermal equilibrium conditions, the complexes are continuously dissociating and forming. The MD simulations are used to calculate the experimental observables related to the phenol hydroxyl stretching mode, i.e., the two dimensional infrared vibrational echo spectrum as a function of time, which directly displays the formation and dissociation of the complex through the growth of off-diagonal peaks, and the linear absorption spectrum, which displays two hydroxyl stretch peaks, one for the complex and one for the free phenol. The results of the simulations are compared to previously reported experimental data and are found to be in quite reasonable agreement. The electronic structure calculations show that the complex is T shaped. The classical potential used for the phenol-benzene interaction in the MD simulations is in good accord with the highest level of the electronic structure calculations. A variety of other features is extracted from the simulations including the relationship between the structure and the projection of the electric field on the hydroxyl group. The fluctuating electric field is used to determine the hydroxyl stretch frequency-frequency correlation function (FFCF). The simulations are also used to examine the number distribution of benzene and CCl4 molecules in the first solvent shell around the phenol. It is found that the distribution is not that of the solvent mole fraction of benzene. There are substantial probabilities of finding a phenol in either a pure benzene environment or a pure CCl4 environment. A conjecture is made that relates the FFCF to the local number of benzene molecules in phenol's first solvent shell.
Theory of the vortex-clustering transition in a confined two-dimensional quantum fluid
Yu, Xiaoquan; Billam, Thomas P.; Nian, Jun; Reeves, Matthew T.; Bradley, Ashton S.
2016-08-01
Clustering of like-sign vortices in a planar bounded domain is known to occur at negative temperature, a phenomenon that Onsager demonstrated to be a consequence of bounded phase space. In a confined superfluid, quantized vortices can support such an ordered phase, provided they evolve as an almost isolated subsystem containing sufficient energy. A detailed theoretical understanding of the statistical mechanics of such states thus requires a microcanonical approach. Here we develop an analytical theory of the vortex clustering transition in a neutral system of quantum vortices confined to a two-dimensional disk geometry, within the microcanonical ensemble. The choice of ensemble is essential for identifying the correct thermodynamic limit of the system, enabling a rigorous description of clustering in the language of critical phenomena. As the system energy increases above a critical value, the system develops global order via the emergence of a macroscopic dipole structure from the homogeneous phase of vortices, spontaneously breaking the Z2 symmetry associated with invariance under vortex circulation exchange, and the rotational SO (2 ) symmetry due to the disk geometry. The dipole structure emerges characterized by the continuous growth of the macroscopic dipole moment which serves as a global order parameter, resembling a continuous phase transition. The critical temperature of the transition, and the critical exponent associated with the dipole moment, are obtained exactly within mean-field theory. The clustering transition is shown to be distinct from the final state reached at high energy, known as supercondensation. The dipole moment develops via two macroscopic vortex clusters and the cluster locations are found analytically, both near the clustering transition and in the supercondensation limit. The microcanonical theory shows excellent agreement with Monte Carlo simulations, and signatures of the transition are apparent even for a modest system of 100
Quantum Computing with Electron Spins in Quantum Dots
Vandersypen, L M K; Van Beveren, L H W; Elzerman, J M; Greidanus, J S; De Franceschi, S; Kouwenhoven, Leo P
2002-01-01
We present a set of concrete and realistic ideas for the implementation of a small-scale quantum computer using electron spins in lateral GaAs/AlGaAs quantum dots. Initialization is based on leads in the quantum Hall regime with tunable spin-polarization. Read-out hinges on spin-to-charge conversion via spin-selective tunneling to or from the leads, followed by measurement of the number of electron charges on the dot via a charge detector. Single-qubit manipulation relies on a microfabricated wire located close to the quantum dot, and two-qubit interactions are controlled via the tunnel barrier connecting the respective quantum dots. Based on these ideas, we have begun a series of experiments in order to demonstrate unitary control and to measure the coherence time of individual electron spins in quantum dots.
Thermoelectric transport through quantum dots
Energy Technology Data Exchange (ETDEWEB)
Merker, Lukas Heinrich
2016-06-30
In this thesis the thermoelectric properties (electrical conductance, Seebeck coefficient and thermal conductance)of quantum dots described by the Anderson impurity model have been investigated by using the numerical renormalization group (NRG) method. In order to make accurate calculations for thermoelectric properties of quantum impurity systems, a number of recent developments and refinements of the NRG have been implemented. These include the z-averaging and Campo discretization scheme, which enable the evaluation of physical quantities on an arbitrary temperature grid and at large discretization parameter Λ and the full density matrix (FDM) approach, which allows a more accurate calculation of spectral functions and transport coefficients. The implementation of the z-averaging and Campo discretization scheme has been tested within a new method for specific heats of quantum impurities. The accuracy of this new method was established by comparison with the numerical solution of the Bethe-ansatz equations for the Anderson model. The FDM approach was implemented and tested within a new approach to the calculation of impurity contributions to the uniform susceptibilities. Within this method a non-negligible contribution from the ''environmental'' degrees of freedom needs to be taken into account to recover the correct susceptibility, as shown by comparison with the Bethe-ansatz approach. An accurate method to calculate the conductance of a quantum dot is implemented, enabling the extraction of the Fermi liquid scaling coefficients c{sub T} and c{sub B} to high accuracy, being able to verify the results of the renormalized super perturbation theory approach (within its regime of validity). The method was generalized to higher order moments of the local level spectral function. This, as well as reduction of the SU(2) code to the U(1) symmetry, enabled the investigation of the effect of a magnetic field on the thermoelectric properties of quantum
Model of tunnelling through periodic array of quantum dots in a magnetic field
Institute of Scientific and Technical Information of China (English)
I.Yu.Popov; S.A.Osipov
2012-01-01
A two-dimensional periodic array of quantum dots with two laterally coupled leads in a magnetic field is considered.The model of electron transport through the system based on the theory of self-adjoint extensions of symmetric operators is suggested.We obtain the formula for the transmission coefficient and investigate its dependence on the magnetic field.
Spectral Gaps of Dirac Operators Describing Graphene Quantum Dots
Benguria, Rafael D.; Fournais, Søren; Stockmeyer, Edgardo; Van Den Bosch, Hanne
2017-06-01
The two-dimensional Dirac operator describes low-energy excitations in graphene. Different choices for the boundary conditions give rise to qualitative differences in the spectrum of the resulting operator. For a family of boundary conditions, we find a lower bound to the spectral gap around zero, proportional to |Ω|-1/2, where {Ω } \\subset R2 is the bounded region where the Dirac operator acts. This family contains the so-called infinite mass and armchair cases used in the physics literature for the description of graphene quantum dots.
Quantum dots with single-atom precision.
Fölsch, Stefan; Martínez-Blanco, Jesús; Yang, Jianshu; Kanisawa, Kiyoshi; Erwin, Steven C
2014-07-01
Quantum dots are often called artificial atoms because, like real atoms, they confine electrons to quantized states with discrete energies. However, although real atoms are identical, most quantum dots comprise hundreds or thousands of atoms, with inevitable variations in size and shape and, consequently, unavoidable variability in their wavefunctions and energies. Electrostatic gates can be used to mitigate these variations by adjusting the electron energy levels, but the more ambitious goal of creating quantum dots with intrinsically digital fidelity by eliminating statistical variations in their size, shape and arrangement remains elusive. We used a scanning tunnelling microscope to create quantum dots with identical, deterministic sizes. By using the lattice of a reconstructed semiconductor surface to fix the position of each atom, we controlled the shape and location of the dots with effectively zero error. This allowed us to construct quantum dot molecules whose coupling has no intrinsic variation but could nonetheless be tuned with arbitrary precision over a wide range. Digital fidelity opens the door to quantum dot architectures free of intrinsic broadening-an important goal for technologies from nanophotonics to quantum information processing as well as for fundamental studies of confined electrons.
Graphene quantum dots derived from carbon fibers.
Peng, Juan; Gao, Wei; Gupta, Bipin Kumar; Liu, Zheng; Romero-Aburto, Rebeca; Ge, Liehui; Song, Li; Alemany, Lawrence B; Zhan, Xiaobo; Gao, Guanhui; Vithayathil, Sajna Antony; Kaipparettu, Benny Abraham; Marti, Angel A; Hayashi, Takuya; Zhu, Jun-Jie; Ajayan, Pulickel M
2012-02-08
Graphene quantum dots (GQDs), which are edge-bound nanometer-size graphene pieces, have fascinating optical and electronic properties. These have been synthesized either by nanolithography or from starting materials such as graphene oxide (GO) by the chemical breakdown of their extended planar structure, both of which are multistep tedious processes. Here, we report that during the acid treatment and chemical exfoliation of traditional pitch-based carbon fibers, that are both cheap and commercially available, the stacked graphitic submicrometer domains of the fibers are easily broken down, leading to the creation of GQDs with different size distribution in scalable amounts. The as-produced GQDs, in the size range of 1-4 nm, show two-dimensional morphology, most of which present zigzag edge structure, and are 1-3 atomic layers thick. The photoluminescence of the GQDs can be tailored through varying the size of the GQDs by changing process parameters. Due to the luminescence stability, nanosecond lifetime, biocompatibility, low toxicity, and high water solubility, these GQDs are demonstrated to be excellent probes for high contrast bioimaging and biosensing applications.
Large quantum dots with small oscillator strength
DEFF Research Database (Denmark)
Stobbe, Søren; Schlereth, T.W.; Höfling, S.
2010-01-01
We have measured the oscillator strength and quantum efficiency of excitons confined in large InGaAs quantum dots by recording the spontaneous emission decay rate while systematically varying the distance between the quantum dots and a semiconductor-air interface. The size of the quantum dots...... is measured by in-plane transmission electron microscopy and we find average in-plane diameters of 40 nm. We have calculated the oscillator strength of excitons of that size assuming a quantum-dot confinement given by a parabolic in-plane potential and a hard-wall vertical potential and predict a very large...... oscillator strength due to Coulomb effects. This is in stark contrast to the measured oscillator strength, which turns out to be so small that it can be described by excitons in the strong confinement regime. We attribute these findings to exciton localization in local potential minima arising from alloy...
Quantum dot devices for optical communications
DEFF Research Database (Denmark)
Mørk, Jesper
2005-01-01
Semiconductor quantum dots are often described as "artificial atoms": They are small nanometre-sized structures in which electrons only are allowed to exist at certain discrete levels due to size quantization, thus allowing the engineering of fundamental properties such as the coupling to light....... The main property of semiconductor quantum dots compared to bulk material or even quantum well structures is the discrete nature of the allowed states, which means that inversion of the medium can be obtained for very low electron densities. This has led to the fabrication of quantum dot lasers with record......-low threshold currents and amplifiers with record-high power levels. In this tutorial we will review the basic properties of quantum dots, emphasizing the properties which are important for laser and amplifier applications, as well as devices for all-optical signal processing. The high-speed properties...
Degenerate ground states and multiple bifurcations in a two-dimensional q-state quantum Potts model.
Dai, Yan-Wei; Cho, Sam Young; Batchelor, Murray T; Zhou, Huan-Qiang
2014-06-01
We numerically investigate the two-dimensional q-state quantum Potts model on the infinite square lattice by using the infinite projected entangled-pair state (iPEPS) algorithm. We show that the quantum fidelity, defined as an overlap measurement between an arbitrary reference state and the iPEPS ground state of the system, can detect q-fold degenerate ground states for the Z_{q} broken-symmetry phase. Accordingly, a multiple bifurcation of the quantum ground-state fidelity is shown to occur as the transverse magnetic field varies from the symmetry phase to the broken-symmetry phase, which means that a multiple-bifurcation point corresponds to a critical point. A (dis)continuous behavior of quantum fidelity at phase transition points characterizes a (dis)continuous phase transition. Similar to the characteristic behavior of the quantum fidelity, the magnetizations, as order parameters, obtained from the degenerate ground states exhibit multiple bifurcation at critical points. Each order parameter is also explicitly demonstrated to transform under the Z_{q} subgroup of the symmetry group of the Hamiltonian. We find that the q-state quantum Potts model on the square lattice undergoes a discontinuous (first-order) phase transition for q=3 and q=4 and a continuous phase transition for q=2 (the two-dimensional quantum transverse Ising model).
Scanning gate microscopy of ultra clean carbon nanotube quantum dots
Xue, Jiamin; Dhall, Rohan; Cronin, Stephen B.; LeRoy, Brian J.
2015-01-01
We perform scanning gate microscopy on individual suspended carbon nanotube quantum dots. The size and position of the quantum dots can be visually identified from the concentric high conductance rings. For the ultra clean devices used in this study, two new effects are clearly identified. Electrostatic screening creates non-overlapping multiple sets of Coulomb rings from a single quantum dot. In double quantum dots, by changing the tip voltage, the interactions between the quantum dots can b...
Quantum dots for terahertz generation
Energy Technology Data Exchange (ETDEWEB)
Liu, H C; Aslan, B; Gupta, J A; Wasilewski, Z R; Aers, G C; SpringThorpe, A J; Buchanan, M [Institute for Microstructural Sciences, National Research Council, Ottawa, K1A 0R6 (Canada)], E-mail: h.c.liu@nrc.ca
2008-09-24
Nanostructures made of semiconductors, such as quantum wells and quantum dots (QD), are well known, and some have been incorporated in practical devices. Here we focus on novel structures made of QDs and related devices for terahertz (THz) generation. Their potential advantages, such as low threshold current density, high characteristic temperature, increased differential gain, etc, make QDs promising candidates for light emitting applications in the THz region. Our idea of using resonant tunneling through QDs is presented, and initial results on devices consisting of self-assembled InAs QDs in an undoped GaAs matrix, with a design incorporating a GaInNAs/GaAs short period superlattice, are discussed. Moreover, shallow impurities are also being explored for possible THz emission: the idea is based on the tunneling through bound states of individual donor or acceptor impurities in the quantum well. Initial results on devices having an AlGaAs/GaAs double-barrier resonant tunneling structure are discussed.
Electronic properties of aperiodic quantum dot chains
Korotaev, P. Yu.; Vekilov, Yu. Kh.; Kaputkina, N. E.
2012-04-01
The electronic spectral and transport properties of aperiodic quantum dot chains are investigated. The systems with singular continuous energy spectrum are considered: Thue-Morse chain, double-periodic chain, Rudin-Shapiro chain. The influence of electronic energy in quantum dot on the spectral properties, band structure, density of states and spectral resistivity, is discussed. Low resistivity regions correspond to delocalized states and these states could be current states. Also we discuss the magnetic field application as the way to tune electronic energy in quantum dot and to obtain metallic or insulating conducting states of the systems.
Amplification Without Inversion in Semiconductor Quantum Dot
Hajibadali, A.; Abbasian, K.; Rostami, A.
In this paper, we have realized amplification without inversion (AWI) in quantum dot (QD). A Y-type four-level system of InxGa1-xN quantum dot has been obtained and investigated for AWI. It has been shown that, with proper setting of control fields' amplitude, we can obtain reasonable gain. With proper setting of phase difference of control fields and probe field, we can obtain considerable gain in resonant wavelength. We have designed this system by solving the Schrödinger-Poisson equations for InxGa1-xN quantum dot in GaN substrate, self-consistently.
Time-bin Entanglement from Quantum Dots
Weihs, Gregor; Predojević, Ana
2016-01-01
The desire to have a source of single entangled photon pairs can be satisfied using single quantum dots as emitters. However, we are not bound to pursue only polarization entanglement, but can also exploit other degrees of freedom. In this chapter we focus on the time degree of freedom, to achieve so-called time-bin entanglement. This requires that we prepare the quantum dot coherently into the biexciton state and also build special interferometers for analysis. Finally this technique can be extended to achieve time-bin and polarization hyper-entanglement from a suitable quantum dot.
Fluorescent Quantum Dots for Biological Labeling
McDonald, Gene; Nadeau, Jay; Nealson, Kenneth; Storrie-Lomardi, Michael; Bhartia, Rohit
2003-01-01
Fluorescent semiconductor quantum dots that can serve as "on/off" labels for bacteria and other living cells are undergoing development. The "on/off" characterization of these quantum dots refers to the fact that, when properly designed and manufactured, they do not fluoresce until and unless they come into contact with viable cells of biological species that one seeks to detect. In comparison with prior fluorescence-based means of detecting biological species, fluorescent quantum dots show promise for greater speed, less complexity, greater sensitivity, and greater selectivity for species of interest. There are numerous potential applications in medicine, environmental monitoring, and detection of bioterrorism.
Designing artificial 2D crystals with site and size controlled quantum dots.
Xie, Xuejun; Kang, Jiahao; Cao, Wei; Chu, Jae Hwan; Gong, Yongji; Ajayan, Pulickel M; Banerjee, Kaustav
2017-08-30
Ordered arrays of quantum dots in two-dimensional (2D) materials would make promising optical materials, but their assembly could prove challenging. Here we demonstrate a scalable, site and size controlled fabrication of quantum dots in monolayer molybdenum disulfide (MoS2), and quantum dot arrays with nanometer-scale spatial density by focused electron beam irradiation induced local 2H to 1T phase change in MoS2. By designing the quantum dots in a 2D superlattice, we show that new energy bands form where the new band gap can be controlled by the size and pitch of the quantum dots in the superlattice. The band gap can be tuned from 1.81 eV to 1.42 eV without loss of its photoluminescence performance, which provides new directions for fabricating lasers with designed wavelengths. Our work constitutes a photoresist-free, top-down method to create large-area quantum dot arrays with nanometer-scale spatial density that allow the quantum dots to interfere with each other and create artificial crystals. This technique opens up new pathways for fabricating light emitting devices with 2D materials at desired wavelengths. This demonstration can also enable the assembly of large scale quantum information systems and open up new avenues for the design of artificial 2D materials.
Ihly, Rachelle
2014-01-01
This thesis explores the understanding of the chemistry and physics of colloidal quantum dots for practical solar energy photoconversion. Solar cell devices that make use of PbS quantum dots generally rely on constant and unchanged optical properties such that band gap energies remain tuned within the device. The design and development of unique experiments to ascertain mechanisms of optical band gap shifts occurring in PbS quantum dot thin-films exposed to air are discussed. The systematic s...
Quantum Dots in Vertical Nanowire Devices
Van Weert, M.
2010-01-01
The research described in this thesis is aimed at constructing a quantum interface between a single electron spin and a photon, using a nanowire quantum dot. Such a quantum interface enables information transfer from a local electron spin to the polarization of a photon for long distance readout.
Non-adiabatic geometrical quantum gates in semiconductor quantum dots
Solinas, P; Zanghì, N; Rossi, F; Solinas, Paolo; Zanardi, Paolo; Zanghì, Nino; Rossi, Fausto
2003-01-01
In this paper we study the implementation of non-adiabatic geometrical quantum gates with in semiconductor quantum dots. Different quantum information enconding/manipulation schemes exploiting excitonic degrees of freedom are discussed. By means of the Aharanov-Anandan geometrical phase one can avoid the limitations of adiabatic schemes relying on adiabatic Berry phase; fast geometrical quantum gates can be in principle implemented
Energy Spectra of Excitons Bound to a Neutral Acceptor in Quantum Dots
Institute of Scientific and Technical Information of China (English)
XIE Wen-Fang
2004-01-01
The energy spectra of the ground state for an exciton (X) trapped by a neutral acceptor (A0) in a quantum dot with a parabolic confinement have been calculated as a function of the electron-to-hole mass ratio σ by using the hyperspherical coordinates. We find that the (A0, X) complex confined in a quantum dot has in general a larger binding energy than those in a two-dimensional quantum well and a three-dimensional bulk semiconductor, and the binding energy decreases with the increase of the electron-to-hole mass ratio.
Single to quadruple quantum dots with tunable tunnel couplings
Energy Technology Data Exchange (ETDEWEB)
Takakura, T.; Noiri, A.; Obata, T.; Yoneda, J.; Yoshida, K. [Department of Applied Physics, University of Tokyo, 7-3-1 Hongo, Bunkyo-ku, Tokyo 113-8656 (Japan); Otsuka, T.; Tarucha, S. [Department of Applied Physics, University of Tokyo, 7-3-1 Hongo, Bunkyo-ku, Tokyo 113-8656 (Japan); RIKEN, Center for Emergent Matter Science, 3-1 Wako-shi, Saitama 351-0198 (Japan)
2014-03-17
We prepare a gate-defined quadruple quantum dot to study the gate-tunability of single to quadruple quantum dots with finite inter-dot tunnel couplings. The measured charging energies of various double dots suggest that the dot size is governed by the gate geometry. For the triple and quadruple dots, we study the gate-tunable inter-dot tunnel couplings. For the triple dot, we find that the effective tunnel coupling between side dots significantly depends on the alignment of the center dot potential. These results imply that the present quadruple dot has a gate performance relevant for implementing spin-based four-qubits with controllable exchange couplings.
Directory of Open Access Journals (Sweden)
Manvir S. Kushwaha
2014-12-01
-Landau level transitions are seen to be forbidden. The spherical quantum dots have an edge over the strictly two-dimensional quantum dots in that the additional (magnetic quantum number makes the physics richer (but complex. A deeper grasp of the Coulomb blockade, quantum coherence, and entanglement can lead to a better insight into promising applications involving lasers, detectors, storage devices, and quantum computing.
Energy Technology Data Exchange (ETDEWEB)
Kushwaha, Manvir S. [Department of Physics and Astronomy, Rice University, P.O. Box 1892, Houston, TX 77251 (United States)
2014-12-15
transitions are seen to be forbidden. The spherical quantum dots have an edge over the strictly two-dimensional quantum dots in that the additional (magnetic) quantum number makes the physics richer (but complex). A deeper grasp of the Coulomb blockade, quantum coherence, and entanglement can lead to a better insight into promising applications involving lasers, detectors, storage devices, and quantum computing.
Quantum Dots Investigated for Solar Cells
Bailey, Sheila G.; Castro, Stephanie L.; Raffaelle, Ryne P.; Hepp, Aloysius F.
2001-01-01
The NASA Glenn Research Center has been investigating the synthesis of quantum dots of CdSe and CuInS2 for use in intermediate-bandgap solar cells. Using quantum dots in a solar cell to create an intermediate band will allow the harvesting of a much larger portion of the available solar spectrum. Theoretical studies predict a potential efficiency of 63.2 percent, which is approximately a factor of 2 better than any state-of-the-art devices available today. This technology is also applicable to thin-film devices--where it offers a potential four-fold increase in power-to-weight ratio over the state of the art. Intermediate-bandgap solar cells require that quantum dots be sandwiched in an intrinsic region between the photovoltaic solar cell's ordinary p- and n-type regions (see the preceding figure). The quantum dots form the intermediate band of discrete states that allow sub-bandgap energies to be absorbed. However, when the current is extracted, it is limited by the bandgap, not the individual photon energies. The energy states of the quantum dot can be controlled by controlling the size of the dot. Ironically, the ground-state energy levels are inversely proportional to the size of the quantum dots. We have prepared a variety of quantum dots using the typical organometallic synthesis routes pioneered by Ba Wendi et al., in the early 1990's. The most studied quantum dots prepared by this method have been of CdSe. To produce these dots, researchers inject a syringe of the desired organometallic precursors into heated triocytlphosphine oxide (TOPO) that has been vigorously stirred under an inert atmosphere (see the following figure). The solution immediately begins to change from colorless to yellow, then orange and red/brown, as the quantum dots increase in size. When the desired size is reached, the heat is removed from the flask. Quantum dots of different sizes can be identified by placing them under a "black light" and observing the various color differences in
Optical anisotropy in vertically coupled quantum dots
DEFF Research Database (Denmark)
Yu, Ping; Langbein, Wolfgang Werner; Leosson, Kristjan;
1999-01-01
We have studied the polarization of surface and edge-emitted photoluminescence (PL) from structures with vertically coupled In0.5Ga0.5As/GaAs quantum dots (QD's) grown by molecular beam epitaxy. The PL polarization is found to be strongly dependent on the number of stacked layers. While single...... number due to increasing dot size....
Double Acceptor Interaction in Semimagnetic Quantum Dot
Directory of Open Access Journals (Sweden)
A. Merwyn Jasper D. Reuben
2011-01-01
Full Text Available The effect of geometry of the semimagnetic Quantum Dot on the Interaction energy of a double acceptor is computed in the effective mass approximation using the variational principle. A peak is observed at the lower dot sizes as a magnetic field is increased which is attributed to the reduction in confinement.
Quantum Dots Coupled to a Superconductor
DEFF Research Database (Denmark)
Jellinggaard, Anders Robert
are tuned electrostatically. This includes tuning the odd occupation of the dot through a quantum phase transition, where it forms a singlet with excitations in the superconductor. We detail the fabrication of these bottom gated devices, which additionally feature ancillary sensor dots connected...
Ge Quantum Dot Infrared Imaging Camera Project
National Aeronautics and Space Administration — Luna Innovations Incorporated proposes to develop a high performance Ge quantum dots-based infrared (IR) imaging camera on Si substrate. The high sensitivity, large...
Chaotic quantum dots with strongly correlated electrons
Shankar, R.
2007-01-01
Quantum dots pose a problem where one must confront three obstacles: randomness, interactions and finite size. Yet it is this confluence that allows one to make some theoretical advances by invoking three theoretical tools: Random Matrix theory (RMT), the Renormalization Group (RG) and the 1/N expansion. Here the reader is introduced to these techniques and shown how they may be combined to answer a set of questions pertaining to quantum dots
Start Shift of Individual Quantum Dots
1999-06-18
We will here describe the results of the influence of electric field on InP quantum dots embedded in GalnP, lattice matched to GaAs. Experimental...details The sample we used was grown by metal-organic vapour phase epitaxy, and contained InP quantum dots in GanP, lattice matched to GaAs (n-type
Germanium quantum dots: Optical properties and synthesis
Heath, James R.; Shiang, J. J.; Alivisatos, A. P.
1994-01-01
Three different size distributions of Ge quantum dots (>~200, 110, and 60 Å) have been synthesized via the ultrasonic mediated reduction of mixtures of chlorogermanes and organochlorogermanes (or organochlorosilanes) by a colloidal sodium/potassium alloy in heptane, followed by annealing in a sealed pressure vessel at 270 °C. The quantum dots are characterized by transmission electron microscopy, x-ray powder diffraction, x-ray photoemission, infrared spectroscopy, and Raman spectroscopy. Col...
Renormalization in Periodically Driven Quantum Dots.
Eissing, A K; Meden, V; Kennes, D M
2016-01-15
We report on strong renormalization encountered in periodically driven interacting quantum dots in the nonadiabatic regime. Correlations between lead and dot electrons enhance or suppress the amplitude of driving depending on the sign of the interaction. Employing a newly developed flexible renormalization-group-based approach for periodic driving to an interacting resonant level we show analytically that the magnitude of this effect follows a power law. Our setup can act as a non-Markovian, single-parameter quantum pump.
Submonolayer Quantum Dot Infrared Photodetector
Ting, David Z.; Bandara, Sumith V.; Gunapala, Sarath D.; Chang, Yia-Chang
2010-01-01
A method has been developed for inserting submonolayer (SML) quantum dots (QDs) or SML QD stacks, instead of conventional Stranski-Krastanov (S-K) QDs, into the active region of intersubband photodetectors. A typical configuration would be InAs SML QDs embedded in thin layers of GaAs, surrounded by AlGaAs barriers. Here, the GaAs and the AlGaAs have nearly the same lattice constant, while InAs has a larger lattice constant. In QD infrared photodetector, the important quantization directions are in the plane perpendicular to the normal incidence radiation. In-plane quantization is what enables the absorption of normal incidence radiation. The height of the S-K QD controls the positions of the quantized energy levels, but is not critically important to the desired normal incidence absorption properties. The SML QD or SML QD stack configurations give more control of the structure grown, retains normal incidence absorption properties, and decreases the strain build-up to allow thicker active layers for higher quantum efficiency.
Quantum dots as biophotonics tools.
Cesar, Carlos L
2014-01-01
This chapter provides a short review of quantum dots (QDs) physics, applications, and perspectives. The main advantage of QDs over bulk semiconductors is the fact that the size became a control parameter to tailor the optical properties of new materials. Size changes the confinement energy which alters the optical properties of the material, such as absorption, refractive index, and emission bands. Therefore, by using QDs one can make several kinds of optical devices. One of these devices transforms electrons into photons to apply them as active optical components in illumination and displays. Other devices enable the transformation of photons into electrons to produce QDs solar cells or photodetectors. At the biomedical interface, the application of QDs, which is the most important aspect in this book, is based on fluorescence, which essentially transforms photons into photons of different wavelengths. This chapter introduces important parameters for QDs' biophotonic applications such as photostability, excitation and emission profiles, and quantum efficiency. We also present the perspectives for the use of QDs in fluorescence lifetime imaging (FLIM) and Förster resonance energy transfer (FRET), so useful in modern microscopy, and how to take advantage of the usually unwanted blinking effect to perform super-resolution microscopy.
Sikkenk, Tycho S.; Coester, Kris; Buhrandt, Stefan; Fritz, Lars; Schmidt, Kai P.
2017-02-01
The classical Ising model on the frustrated three-dimensional (3D) swedenborgite lattice has disordered spin liquid ground states for all ratios of inter- and intraplanar couplings. Quantum fluctuations due to a transverse field give rise to several exotic phenomena. In the limit of weakly coupled kagome layers we find a 3D version of disorder by disorder degeneracy lifting. For large out-of-plane couplings one-dimensional macrospins are formed, which realize a disordered macrospin liquid phase on an emerging two-dimensional triangular lattice. We speculate about a possibly exotic version of quantum criticality that connects the polarized phase to the macrospin liquid.
Quantum mechanical treatment of a constrained particle on two dimensional sphere
Jahangiri, L.; Panahi, H.
2016-12-01
In this work, we study the motion of a particle on two dimensional sphere. By writing the Schrodinger equation, we obtain the wave function and energy spectra for three dimensional harmonic oscillator potential plus trigonometric Rosen-Morse non-central potential. By letting three special cases for intertwining operator, we investigate the energy spectra and wave functions for Smorodinsky-Winternitz potential model.
Quantum-corrected two-dimensional Horava-Lifshitz black hole entropy
Anacleto, M A; Brito, F A; Mota-Silva, J C
2015-01-01
In this paper we focus on the Halmiton-Jacobi method to determine the temperature and the entropy of a two-dimensional Horava-Lifshitz black hole by using the generalized uncertainty principles (GUP). We also address the product of horizons, mainly concerning the event, Cauchy, cosmological and virtual horizons.
Quantum-Corrected Two-Dimensional Horava-Lifshitz Black Hole Entropy
Directory of Open Access Journals (Sweden)
M. A. Anacleto
2016-01-01
Full Text Available We focus on the Hamilton-Jacobi method to determine several thermodynamic quantities such as temperature, entropy, and specific heat of two-dimensional Horava-Lifshitz black holes by using the generalized uncertainty principles (GUP. We also address the product of horizons, mainly concerning the event, Cauchy, and cosmological and virtual horizons.
Coherent electron focusing with quantum point contacts in a two-dimensional electron gas
Houten, H. van; Beenakker, C.W.J.; Williamson, J.G.; Broekaart, M.E.I.; Loosdrecht, P.H.M. van; Wees, B.J. van; Mooij, J.E.; Foxon, C.T.; Harris, J.J.
1989-01-01
Transverse electron focusing in a two-dimensional electron gas is investigated experimentally and theoretically for the first time. A split Schottky gate on top of a GaAs-AlxGa1–xAs heterostructure defines two point contacts of variable width, which are used as injector and collector of ballistic el
Two new integrable cases of two-dimensional quantum mechanics with a magnetic field
Marikhin, V. G.
2016-04-01
Two integrable cases of two-dimensional Schrödinger equation with a magnetic field are proposed. Using the polar coordinates and the symmetrical gauge, we will obtain solutions of these equations through biconfluent and confluent Heun functions. The quantization rules will be derived for both systems under consideration.
Bakke, K.; Belich, H.
2014-07-01
We study the effects of the Lorentz symmetry violation in the nonrelativistic quantum dynamics of a spin-1/2 neutral particle interacting with external fields confined to a two-dimensional quantum ring (W.-C. Tan, J.C. Inkson, Semicond. Sci. Technol. 11, 1635 (1996)). We show a possible scenario for the Lorentz symmetry breaking that permits us to make an analogy with the Landau-Aharonov-Casher system (M. Ericsson, E. Sjöqvist, Phys. Rev. A 65, 013607 (2001)), where a change in the angular frequency characteristic of the confinement of a quantum particle to a two-dimensional ring is obtained. Then, we show that an upper bound for the Lorentz symmetry breaking parameters may be set up. Besides, we analyse another possible scenario of the Lorentz symmetry violation by showing the presence of an analogue of the Coulomb potential. We obtain the bound states solutions to the Schrödinger-Pauli equation and discuss a quantum effect characterized by the dependence of the angular frequency on the quantum numbers of the system.
Quantum Dots in Photonic Crystal Waveguides
DEFF Research Database (Denmark)
Sollner, Immo Nathanael
This Thesis is focused on the study of quantum electrodynamics in photonic crystal waveguides. We investigate the interplay between a single quantum dot and the fundamental mode of the photonic crystal waveguide. We demonstrate experimental coupling eciencies for the spontaneous emission...... into the mode exceeding 98% for emitters spectrally close to the band-edge of the waveguide mode. In addition we illustrate the broadband nature of the underlying eects, by obtaining coupling eciencies above 90% for quantum dots detuned from the band edge by as far as 20nm. These values are in good agreement...... quantum-dot-waveguide coupling. Such a structure is ideally suited for a number of applications in quantum information processing and among others we propose an on-chip spin-photon interface, a single photon transistor, and a deterministic cNOT gate....
Quantum Dots in Photonic Crystal Waveguides
DEFF Research Database (Denmark)
Sollner, Immo Nathanael
This Thesis is focused on the study of quantum electrodynamics in photonic crystal waveguides. We investigate the interplay between a single quantum dot and the fundamental mode of the photonic crystal waveguide. We demonstrate experimental coupling eciencies for the spontaneous emission...... into the mode exceeding 98% for emitters spectrally close to the band-edge of the waveguide mode. In addition we illustrate the broadband nature of the underlying eects, by obtaining coupling eciencies above 90% for quantum dots detuned from the band edge by as far as 20nm. These values are in good agreement...... quantum-dot-waveguide coupling. Such a structure is ideally suited for a number of applications in quantum information processing and among others we propose an on-chip spin-photon interface, a single photon transistor, and a deterministic cNOT gate....
Inter-dot coupling effects on transport through correlated parallel coupled quantum dots
Indian Academy of Sciences (India)
Shyam Chand; G Rajput; K C Sharma; P K Ahluwalia
2009-05-01
Transport through symmetric parallel coupled quantum dot system has been studied, using non-equilibrium Green function formalism. The inter-dot tunnelling with on-dot and inter-dot Coulomb repulsion is included. The transmission coefficient and Landaur–Buttiker like current formula are shown in terms of internal states of quantum dots. The effect of inter-dot tunnelling on transport properties has been explored. Results, in intermediate inter-dot coupling regime show signatures of merger of two dots to form a single composite dot and in strong coupling regime the behaviour of the system resembles the two decoupled dots.
Energy Technology Data Exchange (ETDEWEB)
Weber, Carsten
2008-07-01
This work is focused on the optical dynamics of mesoscopic semiconductor heterostructures, using as prototypes zero-dimensional quantum dots and quantum cascade lasers which consist of quasitwo- dimensional quantum wells. Within a density matrix theory, a microscopic many-particle theory is applied to study scattering effects in these structures: the coupling to external as well as local fields, electron-phonon coupling, coupling to impurities, and Coulomb coupling. For both systems, the investigated effects are compared to experimentally observed results obtained during the past years. In quantum dots, the three-dimensional spatial confinement leads to the necessity to consider a quantum kinetic description of the dynamics, resulting in non-Markovian electron-phonon effects. This can be seen in the spectral phonon sidebands due to interaction with acoustic phonons as well as a damping of nonlinear Rabi oscillations which shows a nonmonotonous intensity and pulse duration dependence. An analysis of the inclusion of the self-interaction of the quantum dot shows that no dynamical local field terms appear for the simple two-level model. Considering local fields which have their origin in many quantum dots, consequences for a two-level quantum dot such as a zero-phonon line broadening and an increasing signal in photon echo experiments are found. For the use of quantum dots in an optical spin control scheme, it is found that the dephasing due to the electron-phonon interaction can be dominant in certain regimes. Furthermore, soliton and breather solutions are studied analytically in nonlinear quantum dot ensembles. Generalizing to quasi-two-dimensional structures, the intersubband dynamics of quantum cascade laser structures is investigated. A dynamical theory is considered in which the temporal evolution of the subband populations and the current density as well as the influence of scattering effects is studied. In the nonlinear regime, the scattering dependence and
Advancements in the Field of Quantum Dots
Mishra, Sambeet; Tripathy, Pratyasha; Sinha, Swami Prasad.
2012-08-01
Quantum dots are defined as very small semiconductor crystals of size varying from nanometer scale to a few micron i.e. so small that they are considered dimensionless and are capable of showing many chemical properties by virtue of which they tend to be lead at one minute and gold at the second minute.Quantum dots house the electrons just the way the electrons would have been present in an atom, by applying a voltage. And therefore they are very judiciously given the name of being called as the artificial atoms. This application of voltage may also lead to the modification of the chemical nature of the material anytime it is desired, resulting in lead at one minute to gold at the other minute. But this method is quite beyond our reach. A quantum dot is basically a semiconductor of very tiny size and this special phenomenon of quantum dot, causes the band of energies to change into discrete energy levels. Band gaps and the related energy depend on the relationship between the size of the crystal and the exciton radius. The height and energy between different energy levels varies inversely with the size of the quantum dot. The smaller the quantum dot, the higher is the energy possessed by it.There are many applications of the quantum dots e.g. they are very wisely applied to:Light emitting diodes: LEDs eg. White LEDs, Photovoltaic devices: solar cells, Memory elements, Biology : =biosensors, imaging, Lasers, Quantum computation, Flat-panel displays, Photodetectors, Life sciences and so on and so forth.The nanometer sized particles are able to display any chosen colour in the entire ultraviolet visible spectrum through a small change in their size or composition.
Quantum Spectra and Classical Orbits in Two-Dimensional Equilateral Triangular Billiards
Institute of Scientific and Technical Information of China (English)
LIN Sheng-Lu; GAO Feng; HONG Zheng-Pin; DU Meng-Li
2005-01-01
@@ We study the correspondence between quantum spectra and classical orbits in the equilateral triangular billiards. The eigenstates of such systems are not separable functions of two variables even though the problem is exactlysolvable. We calculate the Fourier transform of a quantum spectral function and find that the positions of thepeaks match well with the lengths of the classical orbits. This is another example showing that the quantum spectral function provides a bridge between quantum and classical mechanics.
Quantum-dot-in-perovskite solids
Ning, Zhijun
2015-07-15
© 2015 Macmillan Publishers Limited. All rights reserved. Heteroepitaxy - atomically aligned growth of a crystalline film atop a different crystalline substrate - is the basis of electrically driven lasers, multijunction solar cells, and blue-light-emitting diodes. Crystalline coherence is preserved even when atomic identity is modulated, a fact that is the critical enabler of quantum wells, wires, and dots. The interfacial quality achieved as a result of heteroepitaxial growth allows new combinations of materials with complementary properties, which enables the design and realization of functionalities that are not available in the single-phase constituents. Here we show that organohalide perovskites and preformed colloidal quantum dots, combined in the solution phase, produce epitaxially aligned \\'dots-in-a-matrix\\' crystals. Using transmission electron microscopy and electron diffraction, we reveal heterocrystals as large as about 60 nanometres and containing at least 20 mutually aligned dots that inherit the crystalline orientation of the perovskite matrix. The heterocrystals exhibit remarkable optoelectronic properties that are traceable to their atom-scale crystalline coherence: photoelectrons and holes generated in the larger-bandgap perovskites are transferred with 80% efficiency to become excitons in the quantum dot nanocrystals, which exploit the excellent photocarrier diffusion of perovskites to produce bright-light emission from infrared-bandgap quantum-tuned materials. By combining the electrical transport properties of the perovskite matrix with the high radiative efficiency of the quantum dots, we engineer a new platform to advance solution-processed infrared optoelectronics.
Construction of two-dimensional quantum field models through Longo-Witten endomorphisms
Tanimoto, Yoh
2013-01-01
We present a procedure to construct families of local, massive and interacting Haag-Kastler nets on the two-dimensional spacetime through an operator-algebraic method. An existence proof of local observable is given without relying on modular nuclearity. By a similar technique, another family of wedge-local nets is constructed using certain endomorphisms of conformal nets recently studied by Longo and Witten.
Quantum Dots and Their Multimodal Applications: A Review
Holloway, Paul H; Teng-Kuan Tseng; Lei Qian; Debasis Bera
2010-01-01
Semiconducting quantum dots, whose particle sizes are in the nanometer range, have very unusual properties. The quantum dots have band gaps that depend in a complicated fashion upon a number of factors, described in the article. Processing-structure-properties-performance relationships are reviewed for compound semiconducting quantum dots. Various methods for synthesizing these quantum dots are discussed, as well as their resulting properties. Quantum states and confinement of their excitons ...
Phonons in Quantum-Dot Quantum Well
Institute of Scientific and Technical Information of China (English)
QINGuo-Yi
2004-01-01
Phonon modes of A1As/GaAs/A1As and GaAs/A1As/metal Pb quantum-dot quantum wells (QDQW's) with the whole scale up to 90 AО are calculated by using valence force field model (VFFM) based on group theory.Their optical frequency spectra are divided into two nonoverlapping bands, the AlAs-like band and the GaAs-like band,originated from and having frequency interval inside the bulk AlAs optical band and bulk GaAs optical band, respectively.The GaAs-LO (Г)-like modes of QDQW's that have maximum bulk GaAs-LO (Г) parentages in all modes covering thewhole frequency region and all symmetries have always A1 symmetry. Its frequency is controllable by adjusting thestructure parameters. In A1As/GaAs/A1As, it may be controlled to meet any designed frequency in GaAs-like band.The results on GaAs/A1As/metal Pb QDQW's show the same effect of reducing in interface optical phonons by using the metal/semiconductor interface revealed ever by macroscopic model The frequency spectra in both GaAs-like andAlAs-like optical phonon bands are independent of the thickness of Pb shell as long as the thickness of Pb shell is no less than 5 AО Defects at metal/A1As interface have significant influence to AlAs-like optical modes but have only minor influence to GaAs-like optical modes. All these results are important for the studying of the e-ph interaction in QD structures.
Phonons in Quantum-Dot Quantum Well
Institute of Scientific and Technical Information of China (English)
QIN Guo-Yi
2004-01-01
Phonon modes of AlAs/GaAs/AlAs and GaAs/AlAs/metal Pb quantum-dot quantum wells (QDQW's)with the whole scale up to 90 A are calculated by using valence force field model (VFFM) based on group theory.Their optical frequency spectra are divided into two nonoverlapping bands, the AMs-like band and the GaAs-like band,originated from and having frequency interval inside the bulk AlAs optical band and bulk GaAs optical band, respectively.The GaAs-LO (F)-like modes of QDQW's that have maximum bulk GaAs-LO (F) parentages in all modes covering the whole frequency region and all symmetries have always A1 symmetry. Its frequency is controllable by adjusting the structure parameters. In AlAs/GaAs/AlAs, it may be controlled to meet any designed frequency in GaAs-like band.The results on GaAs/AMs/metal Pb QDQW's show the same effect of reducing in interface optical phonons by using the metal/semiconductor interface revealed ever by macroscopic model. The frequency spectra in both GaAs-like and AlAs-like optical phonon bands are independent of the thickness of Pb shell as long as the thickness of Pb shell is no less than 5 A. Defects at metal/AlAs interface have significant influence to AMs-like optical modes but have only minor influence to GaAs-like optical modes. All these results are important for the studying of the e-ph interaction in QD structures.
Electron Spins in Semiconductor Quantum Dots
Hanson, R.
2005-01-01
This thesis describes a series of experiments aimed at understanding and controlling the behavior of the spin degree of freedom of single electrons, confined in semiconductor quantum dots. This research work is motivated by the prospects of using the electron spin as a quantum bit (qubit), the basic
Quantum analysis of plasmonic coupling between quantum dots and nanoparticles
Ahmad, SalmanOgli
2016-10-01
In this study, interaction between core-shells nanoparticles and quantum dots is discussed via the full-quantum-theory method. The electromagnetic field of the nanoparticles is derived by the quasistatic approximation method and the results for different regions of the nanoparticles are quantized from the time-harmonic to the wave equation. Utilizing the optical field quantization, the nanoparticles' and quantum dots' deriving amplitudes contributing to the excitation waves are determined. In the current model, two counterpropagating waves with two different frequencies are applied. We derived the Maxwell-Bloch equations from the Heisenberg-Langevin equations; thus the nanoparticles-quantum dots interaction is perused. Moreover, by full quantum analyzing of the analytical expression, the quantum-plasmonic coupling relation and the Purcell factor are achieved. We show that the spontaneous emission of quantum dots can be dramatically manipulated by engineering the plasmon-plasmon interaction in the core-shells nanoparticles. This issue is a very attractive point for designing a wide variety of quantum-plasmonic sensors. Through the investigation of the nanoparticle plasmonic interaction effects on absorbed power, the results show that the nanoparticles' and quantum dots' absorption saturation state can be switched to each other just by manipulation of their deriving amplitudes. In fact, we manage the interference between the two waves' deriving amplitudes just by the plasmonic interactions effect.
Electromechanical transition in quantum dots
Micchi, G.; Avriller, R.; Pistolesi, F.
2016-09-01
The strong coupling between electronic transport in a single-level quantum dot and a capacitively coupled nanomechanical oscillator may lead to a transition towards a mechanically bistable and blocked-current state. Its observation is at reach in carbon-nanotube state-of-art experiments. In a recent publication [Phys. Rev. Lett. 115, 206802 (2015), 10.1103/PhysRevLett.115.206802] we have shown that this transition is characterized by pronounced signatures on the oscillator mechanical properties: the susceptibility, the displacement fluctuation spectrum, and the ring-down time. These properties are extracted from transport measurements, however the relation between the mechanical quantities and the electronic signal is not always straightforward. Moreover the dependence of the same quantities on temperature, bias or gate voltage, and external dissipation has not been studied. The purpose of this paper is to fill this gap and provide a detailed description of the transition. Specifically we find (i) the relation between the current-noise and the displacement spectrum; (ii) the peculiar behavior of the gate-voltage dependence of these spectra at the transition; (iii) the robustness of the transition towards the effect of external fluctuations and dissipation.
Edén, Mattias
2010-05-01
Three two-dimensional (2D) NMR homonuclear correlation techniques invoking double-quantum (2Q) filtration of the central transitions of half-integer spins are evaluated numerically and experimentally. They correlate directly detected single-quantum (1Q) coherences in the t(2) domain with either of 1Q, two-spin 2Q or single-spin multiple-quantum coherence-evolutions in the indirect (t(1)) dimension. We employ experimental (23)Na and (27)Al NMR on sodium sulfite and the natural mineral sillimanite (SiAl(2)O(5)), in conjunction with simulated 2D spectra from pairs of dipolar-recoupled spins-3/2 and 5/2 at different external magnetic fields, to compare the correlation strategies from the viewpoints of 2D spectral resolution, signal sensitivity, implementational aspects and their relative merits for establishing internuclear proximities and quadrupolar tensor orientations.
Wang, Yunhua; Liu, Yulan; Wang, Biao
2017-01-01
Periodically driven nontrivial quantum states open another door to engineer topological phases in solid systems by light. Here we show, based on the Floquet-Bloch theory, that the on-resonant linearly and circularly polarized infrared light brings in the exotic Floquet quantum spin Hall state and half-metal in two-dimensional Metal-organic frameworks (2D MOFs) because of the unbroken and broken time-reversal symmetry, respectively. We also observe that the off-resonant light triggers topological quantum phase transitions and induces semimetals with pseudospin-1 Dirac-Weyl fermions via the photon-dressed topological band structures of 2D MOFs. This work paves a way to design light-controlled spintronics and optoelectronics based on 2D MOFs. PMID:28134315
Wang, Yunhua; Liu, Yulan; Wang, Biao
2017-01-01
Periodically driven nontrivial quantum states open another door to engineer topological phases in solid systems by light. Here we show, based on the Floquet-Bloch theory, that the on-resonant linearly and circularly polarized infrared light brings in the exotic Floquet quantum spin Hall state and half-metal in two-dimensional Metal-organic frameworks (2D MOFs) because of the unbroken and broken time-reversal symmetry, respectively. We also observe that the off-resonant light triggers topological quantum phase transitions and induces semimetals with pseudospin-1 Dirac-Weyl fermions via the photon-dressed topological band structures of 2D MOFs. This work paves a way to design light-controlled spintronics and optoelectronics based on 2D MOFs.
The quantum spectral analysis of the two-dimensional annular billiard system
Institute of Scientific and Technical Information of China (English)
Zhang Yan-Hui; Zhang Ji-Ouan; Xu Xue-You; Lin Sheng-Lu
2009-01-01
Based on the extended closed-orbit theory together with spectral analysis, this paper studies the correspondence between quantum mechanics and the classical counterpart in a two-dimeusional annular billiard. The results demonstrate that the Fourier-transformed quantum spectra are in very good accordance with the lengths of the classical ballistic trajectories, whereas spectral strength is intimately associated with the shapes of possible open orbits connecting arbitrary two points in the annular cavity. This approach facilitates an intuitive understanding of basic quantum features such as quantum interference, locations of the wavefunctions, and allows quantitative calculations in the range of high energies, where full quantum calculations may become impractical in general. This treatment provides a thread to explore the properties of microjunction transport and even quantum chaos under the much more general system.
Generalized description of few-electron quantum dots at zero and nonzero magnetic fields
Energy Technology Data Exchange (ETDEWEB)
Ciftja, Orion [Department of Physics, Prairie View A and M University, Prairie View, TX 77446 (United States)
2007-01-31
We introduce a generalized ground state variational wavefunction for parabolically confined two-dimensional quantum dots that equally applies to both cases of weak (or zero) and strong magnetic field. The wavefunction has a Laughlin-like form in the limit of infinite magnetic field, but transforms into a Jastrow-Slater wavefunction at zero magnetic field. At intermediate magnetic fields (where a fraction of electrons is spin-reversed) it resembles Halperin's spin-reversed wavefunction for the fractional quantum Hall effect. The properties of this variational wavefunction are illustrated for the case of two-dimensional quantum dot helium (a system of two interacting electrons in a parabolic confinement potential) where we find the description to be an excellent representation of the true ground state for the whole range of magnetic fields.
Dot-in-Well Quantum-Dot Infrared Photodetectors
Gunapala, Sarath; Bandara, Sumith; Ting, David; Hill, cory; Liu, John; Mumolo, Jason; Chang, Yia Chung
2008-01-01
Dot-in-well (DWELL) quantum-dot infrared photodetectors (QDIPs) [DWELL-QDIPs] are subjects of research as potentially superior alternatives to prior QDIPs. Heretofore, there has not existed a reliable method for fabricating quantum dots (QDs) having precise, repeatable dimensions. This lack has constituted an obstacle to the development of uniform, high-performance, wavelength-tailorable QDIPs and of focal-plane arrays (FPAs) of such QDIPs. However, techniques for fabricating quantum-well infrared photodetectors (QWIPs) having multiple-quantum- well (MQW) structures are now well established. In the present research on DWELL-QDIPs, the arts of fabrication of QDs and QWIPs are combined with a view toward overcoming the deficiencies of prior QDIPs. The longer-term goal is to develop focal-plane arrays of radiationhard, highly uniform arrays of QDIPs that would exhibit high performance at wavelengths from 8 to 15 m when operated at temperatures between 150 and 200 K. Increasing quantum efficiency is the key to the development of competitive QDIP-based FPAs. Quantum efficiency can be increased by increasing the density of QDs and by enhancing infrared absorption in QD-containing material. QDIPs demonstrated thus far have consisted, variously, of InAs islands on GaAs or InAs islands in InGaAs/GaAs wells. These QDIPs have exhibited low quantum efficiencies because the numbers of QD layers (and, hence, the areal densities of QDs) have been small typically five layers in each QDIP. The number of QD layers in such a device must be thus limited to prevent the aggregation of strain in the InAs/InGaAs/GaAs non-lattice- matched material system. The approach being followed in the DWELL-QDIP research is to embed In- GaAs QDs in GaAs/AlGaAs multi-quantum- well (MQW) structures (see figure). This material system can accommodate a large number of QD layers without excessive lattice-mismatch strain and the associated degradation of photodetection properties. Hence, this material
Loop equations and Virasoro constraints in non-perturbative two-dimensional quantum gravity
Energy Technology Data Exchange (ETDEWEB)
Dijkgraaf, R.; Verlinde, H. (Princeton Univ., NJ (USA). Joseph Henry Labs.); Verlinde, E. (Institute for Advanced Study, Princeton, NJ (USA). School of Natural Sciences)
1991-01-21
We give a derivation of the loop equation for two-dimensional gravity from the KdV equations and the string equation of the one-matrix model. We find that the loop equation is equivalent to an infinite set of linear constraints on the square root of the partition function satisfying the Virasoro algebra. We give an interpretation of these equations in topological gravity and discuss their extension to multi-matrix models. For the multi-critical models the loop equation naturally singles out the operators corresponding to the primary fields of the minimal models. (orig.).
Loop Equations and Virasoro Constraints in Non-Perturbative Two-Dimensional Quantum Gravity
Dijkgraaf, Robbert; Verlinde, Herman; Verlinde, Erik
We give a derivation of the loop equation for two-dimensional gravity from the KdV equations and the string equation of the one-matrix model. We find that the loop equation is equivalent to an infinite set of linear constraints on the square root of the partition function satisfying the Virasoro algebra. We give an interpretation of these equations in topological gravity and discuss their extension to multi-matrix models. For the multi-critical models the loop equation naturally singles out the operators corresponding to the primary fields of the minimal models.
Institute of Scientific and Technical Information of China (English)
Song Ya-Feng; Lü Yan-Wu; Wen Wei; Liu Xiang-Lin; Yang Shao-Yan; Zhu Qin-Sheng; Wang Zhan-Guo
2012-01-01
The collective charge density excitations in a free-standing nanorod with a two-dimensional parabolic quantum well are investigated within the framework of Bohm-Pine's random-phase approximation in the two-subband model.The new simplified analytical expressions of the Coulomb interaction matrix elements and dielectric functions are derived and numerically discussed.In addition,the electron density and temperature dependences of dispersion features are also investigated.We find that in the two-dimensional parabolic quantum well,the intrasubband upper branch is coupled with the intersubband mode,which is quite different from other quasi-one-dimensional systems like a cylindrical quantum wire with an infinite rectangular potential.In addition,we also find that higher temperature results in the intersubband mode(with an energy of 12 meV(～3 THz))becoming totally damped,which agrees well with the experimental results of Raman scattering in the literature.These interesting properties may provide useful references to the design of free-standing nanorod based devices.
Chern, Li Ern; Hwang, Kyusung; Mizoguchi, Tomonari; Huh, Yejin; Kim, Yong Baek
2017-07-01
The Kagome-lattice-based material, volborthite, Cu3V2O7(OH) 2.2 H2O , has been considered as a promising platform for discovery of unusual quantum ground states due to the frustrated nature of spin interaction. We explore possible quantum spin liquid and magnetically ordered phases in a two-dimensional nonsymmorphic lattice, which is described by the plane group p 2 g g , consistent with the spatial anisotropy of the spin model derived from density functional theory (DFT) for volborthite. Using the projective symmetry group (PSG) analysis and Schwinger boson mean field theory, we classify possible spin liquid phases with bosonic spinons and investigate magnetically ordered phases connected to such states. It is shown, in general, that only translationally invariant mean field spin liquid ansatzes are allowed in two-dimensional nonsymmorphic lattices. We study the mean field phase diagram of the DFT-derived spin model and find that possible quantum spin liquid phases are connected to two types of magnetically ordered phases, a coplanar incommensurate (q ,0 ) spiral order as the ground state and a closely competing coplanar commensurate (π ,π ) spin density wave order. In addition, periodicity enhancement of the two-spinon continuum, a consequence of symmetry fractionalization, is found in the spin liquid state connected to the (π ,π ) spin density wave order. We discuss relevance of these results to recent and future experiments on volborthite.
Topology Change and the Emergence of Geometry in Two Dimensional Causal Quantum Gravity
Westra, W.
2007-01-01
Despite many attempts, gravity has vigorously resisted a unification with the laws of quantum mechanics. Besides a plethora of technical issues, one is also faced with many interesting conceptual problems. The study of quantum gravity in lower dimensional models ameliorates the technical difficultie
Scalable quantum computer architecture with coupled donor-quantum dot qubits
Schenkel, Thomas; Lo, Cheuk Chi; Weis, Christoph; Lyon, Stephen; Tyryshkin, Alexei; Bokor, Jeffrey
2014-08-26
A quantum bit computing architecture includes a plurality of single spin memory donor atoms embedded in a semiconductor layer, a plurality of quantum dots arranged with the semiconductor layer and aligned with the donor atoms, wherein a first voltage applied across at least one pair of the aligned quantum dot and donor atom controls a donor-quantum dot coupling. A method of performing quantum computing in a scalable architecture quantum computing apparatus includes arranging a pattern of single spin memory donor atoms in a semiconductor layer, forming a plurality of quantum dots arranged with the semiconductor layer and aligned with the donor atoms, applying a first voltage across at least one aligned pair of a quantum dot and donor atom to control a donor-quantum dot coupling, and applying a second voltage between one or more quantum dots to control a Heisenberg exchange J coupling between quantum dots and to cause transport of a single spin polarized electron between quantum dots.
Hilbert-Schmidt Geometry of n-Level Jakobczyk-Siennicki Two-Dimensional Quantum Systems
Slater, P B
2005-01-01
Jakobczyk and Siennicki studied two-dimensional sections of a set of Bloch vectors corresponding to n x n density matrices of two-qubit systems (that is, the case n=4). They found essentially five different types of (nontrivial) separability regimes. We compute the Euclidean/Hilbert-Schmidt (HS) separability probabilities assigned to these regimes, and conduct parallel two-dimensional section analyses for the cases n=6,8,9 and 10. We obtain a very wide variety of exact HS-probabilities. For n>6, the probabilities are those of having a partial positive transpose (PPT). For the n=6 case, we also obtain biseparability probabilities; in the n=8,9 instances, bi-PPT probabilities; and for n=8, tri-PPT probabilities. By far, the most frequently recorded probability for n>4 is Pi/4 = 0.785398$. We also conduct a number of related analyses, pertaining to the (one-dimensional) boundaries (both exterior and interior) of the separability and PPT domains, and discuss some exact calculations pertaining to the 9-dimensional...
UV Nano-Lights: Nonlinear Quantum Dot-Plasmon Coupling
2014-08-01
method is also applicable to bare nanoparticles in polar solvents. 15. SUBJECT TERMS Quantum Dots, Nonlinear Optical Materials , Energy...TERMS Quantum Dots, Nonlinear Optical Materials , Energy Conservation, Up-conversion 16. SECURITY CLASSIFICATION OF: 17. LIMITATION OF ABSTRACT
Inorganic passivation and doping control in colloidal quantum dot photovoltaics
Hoogland, Sjoerd H.
2012-01-01
We discuss strategies to reduce midgap trap state densities in colloidal quantum dot films and requirements to control doping type and magnitude. We demonstrate that these improvements result in colloidal quantum dot solar cells with certified 7.0% efficiency.
Energy Technology Data Exchange (ETDEWEB)
Radozycki, Tomasz [Cardinal Stefan Wyszynski University, Faculty of Mathematics and Natural Sciences, College of Sciences, Warsaw (Poland)
2015-09-15
The Lorentz transformation properties of the equal-time bound-state Bethe-Salpeter amplitude in the two-dimensional massless quantum electrodynamics (the so-called Schwinger model) are considered. It is shown that while boosting a bound state (a 'meson') this amplitude is subject to approximate Lorentz contraction. The effect is exact for large separations of constituent particles ('quarks'), while for small distances the deviation is more significant. For this phenomenon to appear, the full function, i.e. with the inclusion of all instanton contributions, has to be considered. The amplitude in each separate topological sector does not exhibit such properties. (orig.)
Energy Technology Data Exchange (ETDEWEB)
Radożycki, Tomasz, E-mail: t.radozycki@uksw.edu.pl [Faculty of Mathematics and Natural Sciences, College of Sciences, Cardinal Stefan Wyszyński University, Wóycickiego 1/3, 01-938, Warsaw (Poland)
2015-09-24
The Lorentz transformation properties of the equal-time bound-state Bethe–Salpeter amplitude in the two-dimensional massless quantum electrodynamics (the so-called Schwinger model) are considered. It is shown that while boosting a bound state (a ‘meson’) this amplitude is subject to approximate Lorentz contraction. The effect is exact for large separations of constituent particles (‘quarks’), while for small distances the deviation is more significant. For this phenomenon to appear, the full function, i.e. with the inclusion of all instanton contributions, has to be considered. The amplitude in each separate topological sector does not exhibit such properties.
A model of the two-dimensional quantum harmonic oscillator in an $AdS_3$ background
Frick, Rudolf
2016-01-01
In this paper we study a model of the two-dimensional quantum harmonic oscillator in a 3-dimensional anti-de Sitter background. We use a generalized Schr\\"odinger picture in which the analogs of the Schr\\"odinger operators of the particle are independent of both the time and the space coordinates in different representations. The spacetime independent operators of the particle induce the Lie algebra of Killing vector fields of the $AdS_3$ spacetime. In this picture, we have a metamorphosis of the Heisenberg's uncertainty relations.
A model of the two-dimensional quantum harmonic oscillator in an AdS{sub 3} background
Energy Technology Data Exchange (ETDEWEB)
Frick, R. [Universitaet zu Koeln, Institut fuer Theoretische Physik, Cologne (Germany)
2016-10-15
In this paper we study a model of the two-dimensional quantum harmonic oscillator in a three-dimensional anti-de Sitter background. We use a generalized Schroedinger picture in which the analogs of the Schroedinger operators of the particle are independent of both the time and the space coordinates in different representations. The spacetime independent operators of the particle induce the Lie algebra of Killing vector fields of the AdS{sub 3} spacetime. In this picture, we have a metamorphosis of the Heisenberg uncertainty relations. (orig.)
Institute of Scientific and Technical Information of China (English)
JI An-Chun; TIAN Guang-Shan
2007-01-01
In the present paper, we investigate the quantum phase transition in a spatially anisotropic antiferromagnetic Heisenberg model of S = 1 with single-ion energy anisotropy. By using the Schwinger boson representation, we calculate the Gaussian correction to the critical value Jc⊥ caused by quantum spin fluctuations. We find that, for the positive single-ion energy, a nonzero value of Jc⊥ is always needed to stabilize the antiferromagnetic long-range order in this model. It resolves a difference among literature and shows clearly that the effect of quantum fluctuations may qualitatively change a result obtained by the mean-field theories on lower-dimensional systems.
Quantum Poincare Section of a Two-Dimensional hamiltonian in a Coherent State Representation
Institute of Scientific and Technical Information of China (English)
金迎新; 贺凯芬
2002-01-01
We study the quantum behaviour of a quasi-integrable Hamiltonian. The unperturbed Hamiltonian displays degeneracies of energy levels, which become avoided crossings under a nonintegrable perturbation. In this twodimensional system, the quantum Poincaré section plot is constructed in the coherent state representation with the restriction that the centres of the wavepackets are confined at the classical surface of constant energy. It is found that the quantum Poincaré section plot obtained in this way provides an evident counterpart of the classical system.
Coherent transport through interacting quantum dots
Energy Technology Data Exchange (ETDEWEB)
Hiltscher, Bastian
2012-10-05
The present thesis is composed of four different works. All deal with coherent transport through interacting quantum dots, which are tunnel-coupled to external leads. There a two main motivations for the use of quantum dots. First, they are an ideal device to study the influence of strong Coulomb repulsion, and second, their discrete energy levels can easily be tuned by external gate electrodes to create different transport regimes. The expression of coherence includes a very wide range of physical correlations and, therefore, the four works are basically independent of each other. Before motivating and introducing the different works in more detail, we remark that in all works a diagrammatic real-time perturbation theory is used. The fermionic degrees of freedom of the leads are traced out and the elements of the resulting reduced density matrix can be treated explicitly by means of a generalized master equation. How this equation is solved, depends on the details of the problem under consideration. In the first of the four works adiabatic pumping through an Aharonov-Bohm interferometer with a quantum dot embedded in each of the two arms is studied. In adiabatic pumping transport is generated by varying two system parameters periodically in time. We consider the two dot levels to be these two pumping parameters. Since they are located in different arms of the interferometer, pumping is a quantum mechanical effect purely relying on coherent superpositions of the dot states. It is very challenging to identify a quantum pumping mechanism in experiments, because a capacitive coupling of the gate electrodes to the leads may yield an undesired AC bias voltage, which is rectified by a time dependent conductance. Therefore, distinguishing features of these two transport mechanisms are required. We find that the dependence on the magnetic field is the key feature. While the pumped charge is an odd function of the magnetic flux, the rectified current is even, at least in
Coherence and dephasing in self-assembled quantum dots
DEFF Research Database (Denmark)
Hvam, Jørn Märcher; Leosson, K.; Birkedal, Dan
2003-01-01
We measured dephasing times in InGaAl/As self-assembled quantum dots at low temperature using degenerate four-wave mixing. At 0K, the coherence time of the quantum dots is lifetime limited, whereas at finite temperatures pure dephasing by exciton-phonon interactions governs the quantum dot...... coherence. The inferred homogeneous line widths are significantly smaller than the line widths usually observed in the photoluminescence from single quantum dots indicating an additional inhomogeneours broadening mechanism in the latter....
Modulation Response of Semiconductor Quantum Dot Nanocavity Lasers
DEFF Research Database (Denmark)
Lorke, Michael; Nielsen, Torben Roland; Mørk, Jesper
2011-01-01
The modulation response of quantum-dot based nanocavity devices is investigated using a semiconductor theory. We show that high modulation bandwidth is achieved even in the presence of inhomogeneous broadening of the quantum dot ensemble.......The modulation response of quantum-dot based nanocavity devices is investigated using a semiconductor theory. We show that high modulation bandwidth is achieved even in the presence of inhomogeneous broadening of the quantum dot ensemble....
Carbon quantum dots and a method of making the same
Energy Technology Data Exchange (ETDEWEB)
Zidan, Ragaiy; Teprovich, Joseph A.; Washington, Aaron L.
2017-08-22
The present invention is directed to a method of preparing a carbon quantum dot. The carbon quantum dot can be prepared from a carbon precursor, such as a fullerene, and a complex metal hydride. The present invention also discloses a carbon quantum dot made by reacting a carbon precursor with a complex metal hydride and a polymer containing a carbon quantum dot made by reacting a carbon precursor with a complex metal hydride.
LUMINESCENCE OF CADMIUM SULFIDE QUANTUM DOTS IN FLUOROPHOSPHATE GLASSES
Z. O. Lipatova; E. V. Kolobkova; V. A. Aseev
2015-01-01
Cadmium sulfide quantum dots are perspective materials in optics, medicine, biology and optoelectronics. Fluorophosphate glasses, doped with cadmium sulfide quantum dots, were examined in the paper. Heat treatment led to the formation of quantum dots with diameters equal to 2.8 nm, 3.0 nm and 3.8 nm. In view of such changes in the quantum dots size the fundamental absorption edge shift and the luminescence band are being displaced to the long wavelengths. Luminescence lifetime has been fou...
Deep Learning the Quantum Phase Transitions in Random Two-Dimensional Electron Systems
Ohtsuki, Tomoki; Ohtsuki, Tomi
2016-12-01
Random electron systems show rich phases such as Anderson insulator, diffusive metal, quantum Hall and quantum anomalous Hall insulators, Weyl semimetal, as well as strong/weak topological insulators. Eigenfunctions of each matter phase have specific features, but owing to the random nature of systems, determining the matter phase from eigenfunctions is difficult. Here, we propose the deep learning algorithm to capture the features of eigenfunctions. Localization-delocalization transition, as well as disordered Chern insulator-Anderson insulator transition, is discussed.
Design of tunneling injection quantum dot lasers
Institute of Scientific and Technical Information of China (English)
JIA Guo-zhi; YAO Jiang-hong; SHU Yong-chun; WANG Zhan-guo
2007-01-01
To implement high quality tunneling injection quantum dot lasers,effects of primary factors on performance of the tunneling injection quantum dot lasers were investigated. The considered factors were tunneling probability,tunneling time and carriers thermal escape time from the quantum well. The calculation results show that with increasing of the ground-state energy level in quantum well,the tunneling probability increases and the tunneling time decreases,while the thermal escape time decreases because the ground-state energy levelis shallower. Longitudinal optical phonon-assisted tunneling can be an effective method to solve the problem that both the tunneling time and the thermal escape time decrease simultaneously with the ground-state energy level increasing in quantum well.
Angiogenic Profiling of Synthesized Carbon Quantum Dots.
Shereema, R M; Sruthi, T V; Kumar, V B Sameer; Rao, T P; Shankar, S Sharath
2015-10-20
A simple method was employed for the synthesis of green luminescent carbon quantum dots (CQDs) from styrene soot. The CQDs were characterized by transmission electron microscopy, X-ray photoelectron spectroscopy, Fourier transform infrared, and Raman spectroscopy. The prepared carbon quantum dots did not show cellular toxicity and could successfully be used for labeling cells. We also evaluated the effects of carbon quantum dots on the process of angiogenesis. Results of a chorioallantoic membrane (CAM) assay revealed the significant decrease in the density of branched vessels after their treatment with CQDs. Further application of CQDs significantly downregulated the expression levels of pro-angiogenic growth factors like VEGF and FGF. Expression of VEGFR2 and levels of hemoglobin were also significantly lower in CAMs treated with CQDs, indicating that the CQDs inhibit angiogenesis. Data presented here also show that CQDs can selectively target cancer cells and therefore hold potential in the field of cancer therapy.
Two-dimensional models as testing ground for principles and concepts of local quantum physics
Schroer, Bert
2006-02-01
In the past two-dimensional models of QFT have served as theoretical laboratories for testing new concepts under mathematically controllable condition. In more recent times low-dimensional models (e.g., chiral models, factorizing models) often have been treated by special recipes in a way which sometimes led to a loss of unity of QFT. In the present work, I try to counteract this apartheid tendency by reviewing past results within the setting of the general principles of QFT. To this I add two new ideas: (1) a modular interpretation of the chiral model Diff( S)-covariance with a close connection to the recently formulated local covariance principle for QFT in curved spacetime and (2) a derivation of the chiral model temperature duality from a suitable operator formulation of the angular Wick rotation (in analogy to the Nelson-Symanzik duality in the Ostertwalder-Schrader setting) for rational chiral theories. The SL (2, Z) modular Verlinde relation is a special case of this thermal duality and (within the family of rational models) the matrix S appearing in the thermal duality relation becomes identified with the statistics character matrix S. The relevant angular "Euclideanization" is done in the setting of the Tomita-Takesaki modular formalism of operator algebras. I find it appropriate to dedicate this work to the memory of J.A. Swieca with whom I shared the interest in two-dimensional models as a testing ground for QFT for more than one decade. This is a significantly extended version of an "Encyclopedia of Mathematical Physics" contribution hep-th/0502125.
Two-dimensional models as testing ground for principles and concepts of local quantum physics
Energy Technology Data Exchange (ETDEWEB)
Schroer, Bert [FU Berlin (Germany). Institut fuer Theoretische Physik
2005-04-15
In the past two-dimensional models of QFT have served as theoretical laboratories for testing new concepts under mathematically controllable condition. In more recent times low-dimensional models (e.g. chiral models, factoring models) often have been treated by special recipes in a way which sometimes led to a loss of unity of QFT. In the present work I try to counteract this apartheid tendency by reviewing past results within the setting of the general principles of QFT. To this I add two new ideas: (1) a modular interpretation of the chiral model Diff(S)-covariance with a close connection to the recently formulated local covariance principle for QFT in curved spacetime and (2) a derivation of the chiral model temperature duality from a suitable operator formulation of the angular Wick rotation (in analogy to the Nelson-Symanzik duality in the Ostertwalder-Schrader setting) for rational chiral theories. The SL(2,Z) modular Verlinde relation is a special case of this thermal duality and (within the family of rational models) the matrix S appearing in the thermal duality relation becomes identified with the statistics character matrix S. The relevant angular 'Euclideanization' is done in the setting of the Tomita-Takesaki modular formalism of operator algebras. I find it appropriate to dedicate this work to the memory of J. A. Swieca with whom I shared the interest in two-dimensional models as a testing ground for QFT for more than one decade. This is a significantly extended version of an 'Encyclopedia of Mathematical Physics' contribution hep-th/0502125. (author)
Bright infrared LEDs based on colloidal quantum-dots
Sun, Liangfeng
2013-01-01
Record-brightness infrared LEDs based on colloidal quantum-dots have been achieved through control of the spacing between adjacent quantum-dots. By tuning the size of quantum-dots, the emission wavelengths can be tuned between 900nm and 1650nm. © 2013 Materials Research Society.
Ihly, Rachelle
This thesis explores the understanding of the chemistry and physics of colloidal quantum dots for practical solar energy photoconversion. Solar cell devices that make use of PbS quantum dots generally rely on constant and unchanged optical properties such that band gap energies remain tuned within the device. The design and development of unique experiments to ascertain mechanisms of optical band gap shifts occurring in PbS quantum dot thin-films exposed to air are discussed. The systematic study of the absorption properties of PbS quantum dot films exposed to air, heat, and UV illumination as a function of quantum dot size has been described. A method to improve the air-stability of films with atomic layer deposition of alumina is demonstrated. Encapsulation of quantum dot films using a protective layer of alumina results in quantum dot solids that maintain tuned absorption for 1000 hours. This thesis focuses on the use of atomic force microscopy and electrical variants thereof to study the physical and electrical characteristics of quantum dot arrays. These types of studies have broad implications in understanding charge transport mechanisms and solar cell device operation, with a particular emphasis on quantum dot transistors and solar cells. Imaging the channel potential of a PbSe quantum dot thin-film in a transistor showed a uniform distribution of charge coinciding with the transistor current voltage characteristics. In a second study, solar cell device operation of ZnO/PbS heterojunction solar cells was investigated by scanning active cross-sections with Kelvin probe microscopy as a function of applied bias, illumination and device architecture. This technique directly provides operating potential and electric field profiles to characterize drift and diffusion currents occurring in the device. SKPM established a field-free region occurring in the quantum dot layer, indicative of diffusion-limited transport. These results provide the path to optimization of
Zeng, Shengwei; Lü, Weiming; Huang, Zhen; Liu, Zhiqi; Han, Kun; Gopinadhan, Kalon; Li, Changjian; Guo, Rui; Zhou, Wenxiong; Ma, Haijiao Harsan; Jian, Linke; Venkatesan, Thirumalai; Ariando
2016-04-26
Electric field effect in electronic double layer transistor (EDLT) configuration with ionic liquids as the dielectric materials is a powerful means of exploring various properties in different materials. Here, we demonstrate the modulation of electrical transport properties and extremely high mobility of two-dimensional electron gas at LaAlO3/SrTiO3 (LAO/STO) interface through ionic liquid-assisted electric field effect. With a change of the gate voltages, the depletion of charge carrier and the resultant enhancement of electron mobility up to 19 380 cm(2)/(V s) are realized, leading to quantum oscillations of the conductivity at the LAO/STO interface. The present results suggest that high-mobility oxide interfaces, which exhibit quantum phenomena, could be obtained by ionic liquid-assisted field effect.
Sandvik, Anders W
2007-06-01
Using ground-state projector quantum Monte Carlo simulations in the valence-bond basis, it is demonstrated that nonfrustrating four-spin interactions can destroy the Néel order of the two-dimensional S=1/2 Heisenberg antiferromagnet and drive it into a valence-bond solid (VBS) phase. Results for spin and dimer correlations are consistent with a single continuous transition, and all data exhibit finite-size scaling with a single set of exponents, z=1, nu=0.78+/-0.03, and eta=0.26+/-0.03. The unusually large eta and an emergent U(1) symmetry, detected using VBS order parameter histograms, provide strong evidence for a deconfined quantum critical point.
Chakrabarti, S; Chatterjee, B; Debbarma, S; Ghatak, K P
2015-09-01
In this paper we study the influence of strong electric field on the two dimensional (2D)effective electron mass (EEM) at the Fermi level in quantum wells of III-V, ternary and quaternary semiconductors within the framework of k x p formalism by formulating a new 2D electron energy spectrum. It appears taking quantum wells of InSb, InAs, Hg(1-x)Cd(x)Te and In(1-x)Ga(x)As(1-y)P(y) lattice matched to InP as examples that the EEM increases with decreasing film thickness, increasing electric field and increases with increasing surface electron concentration exhibiting spikey oscillations because of the crossing over of the Fermi level by the quantized level in quantum wells and the quantized oscillation occurs when the Fermi energy touches the sub-band energy. The electric field makes the mass quantum number dependent and the oscillatory mass introduces quantum number dependent mass anisotropy in addition to energy. The EEM increases with decreasing alloy composition where the variations are totally band structure dependent. Under certain limiting conditions all the results for all the cases get simplified into the well-known parabolic energy bands and thus confirming the compatibility test. The content of this paper finds three applications in the fields of nano-science and technology.
Resonant tunneling in graphene pseudomagnetic quantum dots.
Qi, Zenan; Bahamon, D A; Pereira, Vitor M; Park, Harold S; Campbell, D K; Neto, A H Castro
2013-06-12
Realistic relaxed configurations of triaxially strained graphene quantum dots are obtained from unbiased atomistic mechanical simulations. The local electronic structure and quantum transport characteristics of y-junctions based on such dots are studied, revealing that the quasi-uniform pseudomagnetic field induced by strain restricts transport to Landau level- and edge state-assisted resonant tunneling. Valley degeneracy is broken in the presence of an external field, allowing the selective filtering of the valley and chirality of the states assisting in the resonant tunneling. Asymmetric strain conditions can be explored to select the exit channel of the y-junction.
Cadmium telluride quantum dots advances and applications
Donegan, John
2013-01-01
Optical Properties of Bulk and Nanocrystalline Cadmium Telluride, Núñez Fernández and M.I. VasilevskiyAqueous Synthesis of Colloidal CdTe Nanocrystals, V. Lesnyak, N. Gaponik, and A. EychmüllerAssemblies of Thiol-Capped CdTe Nanocrystals, N. GaponikFörster Resonant Energy Transfer in CdTe Nanocrystal Quantum Dot Structures, M. Lunz and A.L. BradleyEmission of CdTe Nanocrystals Coupled to Microcavities, Y.P. Rakovich and J.F. DoneganBiological Applications of Cadmium Telluride Semiconductor Quantum Dots, A. Le Cign
Bilayer graphene quantum dot defined by topgates
Energy Technology Data Exchange (ETDEWEB)
Müller, André; Kaestner, Bernd; Hohls, Frank; Weimann, Thomas; Pierz, Klaus; Schumacher, Hans W., E-mail: hans.w.schumacher@ptb.de [Physikalisch-Technische Bundesanstalt, Bundesallee 100, 38116 Braunschweig (Germany)
2014-06-21
We investigate the application of nanoscale topgates on exfoliated bilayer graphene to define quantum dot devices. At temperatures below 500 mK, the conductance underneath the grounded gates is suppressed, which we attribute to nearest neighbour hopping and strain-induced piezoelectric fields. The gate-layout can thus be used to define resistive regions by tuning into the corresponding temperature range. We use this method to define a quantum dot structure in bilayer graphene showing Coulomb blockade oscillations consistent with the gate layout.
Quantum limit for two-dimensional resolution of two incoherent optical point sources
Ang, Shan Zheng; Tsang, Mankei
2016-01-01
We obtain the multiple-parameter quantum Cram\\'er-Rao bound for estimating the Cartesian components of the centroid and separation of two incoherent optical point sources using an imaging system with finite spatial bandwidth. Under quite general and realistic assumptions on the point-spread function of the imaging system, and for weak source strengths, we show that the Cram\\'er-Rao bounds for the x and y components of the separation are independent of the values of those components, which may be well-below the conventional Rayleigh resolution limit. We also propose two linear optics-based measurement methods that approach the quantum bound for the estimation of the Cartesian components of the separation once the centroid has been located. One of the methods is an interferometric scheme that approaches the quantum bound for sub-Rayleigh separations. The other method uses fiber coupling to attain the bound regardless of the distance between the two sources.
High resolution STEM of quantum dots and quantum wires
DEFF Research Database (Denmark)
Kadkhodazadeh, Shima
2013-01-01
This article reviews the application of high resolution scanning transmission electron microscopy (STEM) to semiconductor quantum dots (QDs) and quantum wires (QWRs). Different imaging and analytical techniques in STEM are introduced and key examples of their application to QDs and QWRs...
THz quantum-confined Stark effect in semiconductor quantum dots
DEFF Research Database (Denmark)
Turchinovich, Dmitry; Monozon, Boris S.; Livshits, Daniil A.;
2012-01-01
We demonstrate an instantaneous all-optical manipulation of optical absorption at the ground state of InGaAs/GaAs quantum dots (QDs) via a quantum-confined Stark effect (QCSE) induced by the electric field of incident THz pulses with peak electric fields reaching 200 kV/cm in the free space...
A Polaron in a Quantum Dot Quantum Well
Institute of Scientific and Technical Information of China (English)
ZHANG Li; XIE HongJing; CHEN ChuanYu
2002-01-01
The polaron effect in a quantum dot quantum well (QDQW)system is investigated by using the perturbation method. Both the bound electron states outside and inside the shell well are taken into account . Numerical calculation on the CdS/HgS QDQW shows that the phonon correction to the electron ground state energy is quite significant and cannot be neglected.
Spin correlations in the two-dimensional quantum s=1/2 XY model
Sznajd, J.
1995-08-01
A quantum version of the Niemeijer-van Leeuwen real-space renormalization-group method is used to study the temperature dependence of the two- and four-spin correlations in the quantum XY model on the triangular lattice. The first-order cumulant expansion results suggest, similarly to other methods, a low-temperature phase of an essentially different kind from that predicted for the classical model. The possible explanation of the origin of the spurious 2D Heisenberg-like nontrivial fixed point in some renormalization-group calculations is also proposed.
Two-Dimensional GaAs/AlGaAs Multiple Quantum Well Spatial Light Modulators
Institute of Scientific and Technical Information of China (English)
Qin Wang; Jan Borglind; Smilja Becanovic; Stéphane Junique; Daniel (A)gren; Bertrand Noharet; Linda H(o)glund; Olof (O)berg; Erik Petrini; Jan Y. Andersson; Hedda Malm
2003-01-01
Multiple quantum well spatial light modulators with 128x128 array in 38μm pitch are fabricated using two pproaches, one with an attachment of an optical substrate and another one without. These two fabrication processes are described and compared.
Two-dimensional time-dependent quantum-mechanical scattering event
Energy Technology Data Exchange (ETDEWEB)
Galbraith, I.; Ching, Y.S.; Abraham, E.
1984-01-01
Nonrelativistic quantum-mechanical scattering in two dimensions is studied numerically by integrating the time-dependent Schroedinger equation. A partial-wave analysis is used to discuss the numerical results. A potential barrier, a square well and a single slit are considered as the scattering potentials.
Quantum ratchet effects induced by terahertz radiation in GaN-based two-dimensional structures
Weber, W.; Golub, L. E.; Danilov, S. N.; Karch, J.; Reitmaier, C.; Wittmann, B.; Bel' kov, V. V.; Ivchenko, E. L.; Kvon, Z. D.; Vinh, N. Q.; van der Meer, A. F. G.; Murdin, B.; Ganichev, S. D.
2008-01-01
Photogalvanic effects are observed and investigated in wurtzite (0001)-oriented GaN/AlGaN low-dimensional structures excited by terahertz radiation. The structures are shown to represent linear quantum ratchets. Experimental and theoretical analysis exhibits that the observed photocurrents are relat
Quantum ratchet effects induced by terahertz radiation in GaN-based two-dimensional structures
Weber, W.; Golub, L. E.; Danilov, S. N.; Karch, J.; Reitmaier, C.; Wittmann, B.; Bel'Kov, V. V.; Ivchenko, E. L.; Kvon, Z. D.; Vinh, N. Q.; van der Meer, A. F. G.; Murdin, B.; Ganichev, S. D.
2008-06-01
Photogalvanic effects are observed and investigated in wurtzite (0001)-oriented GaN/AlGaN low-dimensional structures excited by terahertz radiation. The structures are shown to represent linear quantum ratchets. Experimental and theoretical analysis exhibits that the observed photocurrents are related to the lack of an inversion center in the GaN-based heterojunctions.
Probing silicon quantum dots by single-dot techniques
Sychugov, Ilya; Valenta, Jan; Linnros, Jan
2017-02-01
Silicon nanocrystals represent an important class of non-toxic, heavy-metal free quantum dots, where the high natural abundance of silicon is an additional advantage. Successful development in mass-fabrication, starting from porous silicon to recent advances in chemical and plasma synthesis, opens up new possibilities for applications in optoelectronics, bio-imaging, photovoltaics, and sensitizing areas. In this review basic physical properties of silicon nanocrystals revealed by photoluminescence spectroscopy, lifetime, intensity trace and electrical measurements on individual nanoparticles are summarized. The fabrication methods developed for accessing single Si nanocrystals are also reviewed. It is concluded that silicon nanocrystals share many of the properties of direct bandgap nanocrystals exhibiting sharp emission lines at low temperatures, on/off blinking, spectral diffusion etc. An analysis of reported results is provided in comparison with theory and with direct bandgap material quantum dots. In addition, the role of passivation and inherent interface/matrix defects is discussed.
Jug, Giancarlo; Ziegler, Klaus
1997-10-01
We present a calculation for the second moment of the local density of states in a model of a two-dimensional quantum dot array near the quantum Hall transition. The quantum dot array model is a realistic adaptation of the lattice model for the quantum Hall transition in the two-dimensional electron gas in an external magnetic field proposed by Ludwig, Fisher, Shankar, and Grinstein. We make use of a Dirac fermion representation for the Green's functions in the presence of fluctuations for the quantum dot energy levels. A saddle-point approximation yields nonperturbative results for the first and second moments of the local density of states, showing interesting fluctuation behavior near the quantum Hall transition. To our knowledge we discuss here one of the first analytic characterizations of chaotic behavior for a two-dimensional mesoscopic structure. The connection with possible experimental investigations of the local density of states in the quantum dot array structures (by means of NMR Knight-shift or single-electron-tunneling techniques) and our work is also established.
Spin-zero anomaly in the magnetic quantum oscillations of a two-dimensional metal
Energy Technology Data Exchange (ETDEWEB)
Wosnitza, J; Ignatchik, O; Bergk, B [Hochfeld-Magnetlabor Dresden (HLD), Forschungszentrum Dresden-Rossendorf, D-01314 Dresden (Germany); Gvozdikov, V M [Max-Planck-Institut fuer Physik komplexer Systeme, D-01187 Dresden (Germany); Hagel, J [Institut fuer Festkoerperphysik, Technische Universitaet Dresden, D-01062 Dresden (Germany); Meeson, P J [H H Wills Physics Laboratory, University of Bristol, Bristol BS8 1TL (United Kingdom); Schlueter, J A [Materials Science Division, Argonne National Laboratory, Argonne, IL 60439 (United States); Davis, H; Winter, R W; Gard, G L [Department of Chemistry, Portland State University, Portland, OR 97207 (United States)], E-mail: J.Wosnitza@fzd.de
2008-08-15
We report on an anomalous behavior of the spin-splitting zeros in the de Haas-van Alphen (dHvA) signal of a quasi-two-dimensional organic superconductor. The zeros as well as the angular dependence of the amplitude of the second harmonic deviate remarkably from the standard Lifshitz-Kosevich (LK) prediction. In contrast, the angular dependence of the fundamental dHvA amplitude as well as the spin-splitting zeros of the Shubnikov-de Haas (SdH) signal follow the LK theory. We can explain this behavior of the dHvA signal by small chemical-potential (CP) oscillations and find a very good agreement between theory and experiment. A detailed wave-shape analysis of the dHvA oscillations corroborates the existence of an oscillating CP. We discuss the absence of the above spin-zero effect in the SdH signal and argue that in {beta}-prime-(BEDT-TTF){sub 2}SF{sub 5}CH{sub 2}CF{sub 2}SO{sub 3} it can be explained by an incoherent variable range hopping interlayer transport which is insensitive to the small CP oscillations.
Spin-zero anomaly in the magnetic quantum oscillations of a two-dimensional metal.
Energy Technology Data Exchange (ETDEWEB)
Wosnitza, J.; Gvozdikov, V. M.; Hagel, J.; Meeson, P. J.; Schlueter, J. A.; Ignatchick, O.; Winter, R. W.; Gard, G. L.; Davis, H.; Bergk, B.; Materials Science Division; Technische Univ. Dresden; Max-Planck Inst. Phys. Complex Systems; Univ. Bristol; Portland State Univ.
2008-01-01
We report on an anomalous behavior of the spin-splitting zeros in the de Haas-van Alphen (dHvA) signal of a quasi-two-dimensional organic superconductor. The zeros as well as the angular dependence of the amplitude of the second harmonic deviate remarkably from the standard Lifshitz-Kosevich (LK) prediction. In contrast, the angular dependence of the fundamental dHvA amplitude as well as the spin-splitting zeros of the Shubnikov-de Haas (SdH) signal follow the LK theory. We can explain this behavior of the dHvA signal by small chemical-potential (CP) oscillations and find a very good agreement between theory and experiment. A detailed wave-shape analysis of the dHvA oscillations corroborates the existence of an oscillating CP. We discuss the absence of the above spin-zero effect in the SdH signal and argue that in {beta}{double_prime}-(BEDT-TTF){sub 2}SF{sub 5}CH{sub 2}CF{sub 2}SO{sub 3} it can be explained by an incoherent variable range hopping interlayer transport which is insensitive to the small CP oscillations.
Two-dimensional models as testing ground for principles and concepts of local quantum physics
Schrör, B
2005-01-01
In the past two-dimensional models of QFT have served as theoretical laboratories for testing new concepts under mathematically controllable condition. In more recent times low-dimensional models (e.g. chiral models, factorizing models) often have been treated by special recipes in a way which sometimes led to a loss of unity of QFT. In the present work I try to counteract this apartheid tendency by reviewing past results within the setting of the general principles of QFT. To this I add two new ideas: a derivation of the chiral model temperature duality from a suitable operator formulation of the angular Wick rotation (in analogy to the Nelson-Symanzik duality in the Ostertwalder-Schrader setting) and a modular interpretation of the chiral model Diff(S)-covariance with a close connection to the recently formulated local covariance principle for QFT in curved spacetime. As a special case of the thermal duality, the SL(2,Z) modular Verlinde relation is thus a consequence of the principles of thermal QFT togeth...
Ground-state properties of two-dimensional quantum fluid helium and hydrogen mixtures
Um, C I; Oh, H G
1998-01-01
Using a variational Jastrow wavefunction extended to include a three-body correlation function and a hypernetted chain scheme with the contributions of elementary diagrams, we analyze the ground-state energies and the structural properties of two-dimensional H- sup 4 He and H sub 2 - sup 4 He mixtures. The mixtures are in equilibrium at a lower density compared to a pure sup 4 He system because of the large zero-point energies of the hydrogen atom and molecule. We evaluate the lowering of the ground-state energies as a function of the impurity concentration and total density of mixtures. Comparing the result with boson sup 3 He- sup 4 He mixtures, we show that the shifts of energy mainly come from the difference of the zero-point energies of the impurities rather than from the interatomic potentials.We also analyze the enthalpies to study the miscibility and conclude that boson-boson mixtures are completely phase separated in their equilibria.
Local Gate Control of a Carbon Nanotube Double Quantum Dot
2016-04-04
Nanotube Double Quantum Dot N. Mason,*† M. J. Biercuk,* C. M. Marcus† We have measured carbon nanotube quantum dots with multiple electro- static gates and...used the resulting enhanced control to investigate a nano- tube double quantum dot. Transport measurements reveal honeycomb charge stability diagrams...This ability to control electron interactions in the quantum regime in a molecular conductor is important for applications such as quantum
Imaging and Manipulating Energy Transfer Among Quantum Dots at Individual Dot Resolution.
Nguyen, Duc; Nguyen, Huy A; Lyding, Joseph W; Gruebele, Martin
2017-06-27
Many processes of interest in quantum dots involve charge or energy transfer from one dot to another. Energy transfer in films of quantum dots as well as between linked quantum dots has been demonstrated by luminescence shift, and the ultrafast time-dependence of energy transfer processes has been resolved. Bandgap variation among dots (energy disorder) and dot separation are known to play an important role in how energy diffuses. Thus, it would be very useful if energy transfer could be visualized directly on a dot-by-dot basis among small clusters or within films of quantum dots. To that effect, we report single molecule optical absorption detected by scanning tunneling microscopy (SMA-STM) to image energy pooling from donor into acceptor dots on a dot-by-dot basis. We show that we can manipulate groups of quantum dots by pruning away the dominant acceptor dot, and switching the energy transfer path to a different acceptor dot. Our experimental data agrees well with a simple Monte Carlo lattice model of energy transfer, similar to models in the literature, in which excitation energy is transferred preferentially from dots with a larger bandgap to dots with a smaller bandgap.
Correlation of Conductance Measurements from a Quantum Dot with Three Terminals
Toonen, Ryan; Prada, Marta; Qin, Hua; Huettel, Andreas; Goswami, Srijit; Blick, Robert; Eberl, Karl
2005-03-01
We have measured the differential conductance of a quantum dot coupled by three tunable tunneling barriers to three terminals. The quantum dot is formed by laterally constricting a two-dimensional electron gas (2DEG) in an AlxGa1-xAs/GaAs heterostructure with Schottky split-gates. The advantage to performing conductance measurements on a quantum dot with three leads is that we are able to directly measure information about the individual tunneling barriers and determine how the states interact with the leads. At a base temperature of 250mK, we have observed new phenomena not previously reported from three-terminal, mesoscopic experiments. These effects include conductance peak suppression in the nonlinear bias regime and the simultaneous coupling of two different states to two separate leads.
Single-particle tracking of quantum dot-conjugated prion proteins inside yeast cells
Energy Technology Data Exchange (ETDEWEB)
Tsuji, Toshikazu; Kawai-Noma, Shigeko [Department of Biomolecular Engineering, Graduate School of Biosciences and Biotechnology, Tokyo Institute of Technology, B56, 4259 Nagatsuta, Midori-ku, Yokohama 226-8501 (Japan); Pack, Chan-Gi [Cellular Informatics Laboratory, RIKEN Advanced Science Institute, Wako-shi, Saitama 351-0198 (Japan); Terajima, Hideki [Department of Biomolecular Engineering, Graduate School of Biosciences and Biotechnology, Tokyo Institute of Technology, B56, 4259 Nagatsuta, Midori-ku, Yokohama 226-8501 (Japan); Yajima, Junichiro; Nishizaka, Takayuki [Department of Physics, Gakushuin University, 1-5-1 Mejiro, Toshima-ku, Tokyo 171-8588 (Japan); Kinjo, Masataka [Laboratory of Molecular Cell Dynamics, Graduate School of Life Sciences, Hokkaido University, Sapporo 001-0021 (Japan); Taguchi, Hideki, E-mail: taguchi@bio.titech.ac.jp [Department of Biomolecular Engineering, Graduate School of Biosciences and Biotechnology, Tokyo Institute of Technology, B56, 4259 Nagatsuta, Midori-ku, Yokohama 226-8501 (Japan)
2011-02-25
Research highlights: {yields} We develop a method to track a quantum dot-conjugated protein in yeast cells. {yields} We incorporate the conjugated quantum dot proteins into yeast spheroplasts. {yields} We track the motions by conventional or 3D tracking microscopy. -- Abstract: Yeast is a model eukaryote with a variety of biological resources. Here we developed a method to track a quantum dot (QD)-conjugated protein in the budding yeast Saccharomyces cerevisiae. We chemically conjugated QDs with the yeast prion Sup35, incorporated them into yeast spheroplasts, and tracked the motions by conventional two-dimensional or three-dimensional tracking microscopy. The method paves the way toward the individual tracking of proteins of interest inside living yeast cells.
Liu, Chieh-Wen; Liu, Chieh-I.; Liang, C.-T.; Kim, Gil-Ho; Huang, C. F.; Hang, D. R.; Chang, Y. H.; Ritchie, D. A.
2017-08-01
Temperature-driven flow lines are studied in the conductivity plane in a GaAs-based two-dimensional electron system containing self-assembled InAs dots when Landau level filling factor ν = 2-4. In the insulator-quantum Hall (I-QH) transition resulting from the floating-up of the extended states, the flow diagram shows the critical behavior and we observed the expected semicircle in the strongest disorder case. By decreasing the effective disorder, we find that such flow lines can leave the I-QH regime and correspond to the plateau-plateau transition between ν = 4 and 2. The evolution of the conductivity curve at low magnetic fields demonstrates the importance of Landau-level mixing to the semicircle when the extended states float up.
Photoluminescence studies of single InGaAs quantum dots
DEFF Research Database (Denmark)
Leosson, Kristjan; Jensen, Jacob Riis; Hvam, Jørn Märcher
1999-01-01
Semiconductor quantum dots are considered a promising material system for future optical devices and quantum computers. We have studied the low-temperature photoluminescence properties of single InGaAs quantum dots embedded in GaAs. The high spatial resolution required for resolving single dots...... to resolve luminescence lines from individual quantum dots, revealing an atomic-like spectrum of sharp transition lines. A parameter of fundamental importance is the intrinsic linewidth of these transitions. Using high-resolution spectroscopy we have determined the linewidth and investigated its dependence...... on temperature, which gives information about how the exciton confined to the quantum dot interacts with the surrounding lattice....
Germanium quantum dots: Optical properties and synthesis
Heath, James R.; Shiang, J. J.; Alivisatos, A. P.
1994-07-01
Three different size distributions of Ge quantum dots (≳200, 110, and 60 Å) have been synthesized via the ultrasonic mediated reduction of mixtures of chlorogermanes and organochlorogermanes (or organochlorosilanes) by a colloidal sodium/potassium alloy in heptane, followed by annealing in a sealed pressure vessel at 270 °C. The quantum dots are characterized by transmission electron microscopy, x-ray powder diffraction, x-ray photoemission, infrared spectroscopy, and Raman spectroscopy. Colloidal suspensions of these quantum dots were prepared and their extinction spectra are measured with ultraviolet/visible (UV/Vis) and near infrared (IR) spectroscopy, in the regime from 0.6 to 5 eV. The optical spectra are correlated with a Mie theory extinction calculation utilizing bulk optical constants. This leads to an assignment of three optical features to the E(1), E(0'), and E(2) direct band gap transitions. The E(0') transitions exhibit a strong size dependence. The near IR spectra of the largest dots is dominated by E(0) direct gap absorptions. For the smallest dots the near IR spectrum is dominated by the Γ25→L indirect transitions.
Nonlocal quantum cloning via quantum dots trapped in distant cavities
Institute of Scientific and Technical Information of China (English)
Yu Tao; Zhu Ai-Dong; Zhang Shou
2012-01-01
A scheme for implementing nonlocal quantum cloning via quantum dots trapped in cavities is proposed.By modulating the parameters of the system,the optimal 1 → 2 universal quantum cloning machine,1 → 2 phase-covariant cloning machine,and 1 → 3 economical phase-covariant cloning machine are constructed.The present scheme,which is attainable with current technology,saves two qubits compared with previous cloning machines.
General model for a entanglement-enhanced composed quantum game on a two-dimensional lattice
Miszczak, Jarosław Adam; Sładkowski, Jan
2013-01-01
We introduce a method of analyzing entanglement enhanced quantum games on regular lattices of agents. Our method is valid for setups with periodic and non-periodic boundary conditions. To demonstrate our approach we study two different types games, namely the prisoner's dilemma game and a cooperative Parrondo's game. In both cases we obtain results showing, that entanglement is a crucial resource necessary for the agents to achieve positive capital gain.
Sarkar, Subhajit; Chaudhury, Ranjan; Paul, Samir K.
2017-01-01
The available results from the inelastic neutron scattering experiment performed on the quasi-two dimensional spin 1/2 anti-ferromagnetic material La2CuO4 have been analysed theoretically. The formalism of ours is based on a semi-classical like treatment involving a model of an ideal gas of mobile vortices and anti-vortices built on the background of the Néel state, using the bipartite classical spin configuration corresponding to an XY-anisotropic Heisenberg anti-ferromagnet on a square lattice. The results for the integrated intensities for our spin 1/2 model corresponding to different temperatures, show occurrence of vigorous unphysical oscillations, when convoluted with a realistic spectral window function. These results indicate failure of the conventional semi-classical theoretical model of ideal vortex/anti-vortex gas arising in the Berezinskii-Kosterlitz-Thouless theory for the low spin magnetic systems. A full fledged quantum mechanical formalism and calculations seem crucial for the understanding of topological excitations in such low spin systems. Furthermore, a severe disagreement is found to occur at finite values of energy transfer between the integrated intensities obtained theoretically from the conventional formalism and those obtained experimentally. This further suggests strongly that the full quantum treatment should also incorporate the interaction between the fragile-magnons and the topological excitations. This is quite plausible in view of the recent work establishing such a process in XXZ quantum ferromagnet on 2D lattice. The high spin XXZ quasi-two dimensional antiferromagnet like MnPS3 however follows the conventional theory quite well.
Quantum critical response function in quasi-two-dimensional itinerant antiferromagnets
Varma, C. M.; Zhu, Lijun; Schröder, Almut
2015-10-01
We reexamine the experimental results for the magnetic response function χ''(q ,E ,T ) for q around the antiferromagnetic vectors Q , in the quantum-critical region, obtained by inelastic neutron scattering, on an Fe-based superconductor and on a heavy-fermion compound. The motivation is to compare the results with a recent theory, which shows that the fluctuations in a generic antiferromagnetic model for itinerant fermions map to those in the universality class of the dissipative quantum-XY model. The quantum-critical fluctuations in this model, in a range of parameters, are given by the correlations of spatial and temporal topological defects. The theory predicts a χ''(q ,E ,T ) (i) which is a separable function of (q -Q ) and of (E ,T ) , (ii) at criticality, the energy-dependent part is ∝tanh(E /2 T ) below a cutoff energy, (iii) the correlation time departs from its infinite value at criticality on the disordered side by an essential singularity, and (iv) the correlation length depends logarithmically on the correlation time, so that the dynamical critical exponent z is ∞ . The limited existing experimental results are found to be consistent with the first two unusual predictions from which the linear dependence of the resistivity on T and the T lnT dependence of the entropy also follow. More experiments are suggested, especially to test the theory of variations on the correlation time and length on the departure from criticality.
Otsuka, Yuichi; Yunoki, Seiji; Sorella, Sandro
2016-01-01
The metal-insulator transition has been a subject of intense research since Mott first proposed that the metallic behavior of interacting electrons could turn to an insulating one as electron correlations increase. Here, we consider electrons with massless Dirac-like dispersion in two spatial dimensions, described by the Hubbard models on two geometrically different lattices, and perform numerically exact calculations on unprecedentedly large systems that, combined with a careful finite-size scaling analysis, allow us to explore the quantum critical behavior in the vicinity of the interaction-driven metal-insulator transition. Thereby, we find that the transition is continuous, and we determine the quantum criticality for the corresponding universality class, which is described in the continuous limit by the Gross-Neveu model, a model extensively studied in quantum field theory. Furthermore, we discuss a fluctuation-driven scenario for the metal-insulator transition in the interacting Dirac electrons: The metal-insulator transition is triggered only by the vanishing of the quasiparticle weight, not by the Dirac Fermi velocity, which instead remains finite near the transition. This important feature cannot be captured by a simple mean-field or Gutzwiller-type approximate picture but is rather consistent with the low-energy behavior of the Gross-Neveu model.
Efficient Blue Electroluminescence Using Quantum-Confined Two-Dimensional Perovskites.
Kumar, Sudhir; Jagielski, Jakub; Yakunin, Sergii; Rice, Peter; Chiu, Yu-Cheng; Wang, Mingchao; Nedelcu, Georgian; Kim, Yeongin; Lin, Shangchao; Santos, Elton J G; Kovalenko, Maksym V; Shih, Chih-Jen
2016-10-03
Solution-processed hybrid organic-inorganic lead halide perovskites are emerging as one of the most promising candidates for low-cost light-emitting diodes (LEDs). However, due to a small exciton binding energy, it is not yet possible to achieve an efficient electroluminescence within the blue wavelength region at room temperature, as is necessary for full-spectrum light sources. Here, we demonstrate efficient blue LEDs based on the colloidal, quantum-confined 2D perovskites, with precisely controlled stacking down to one-unit-cell thickness (n = 1). A variety of low-k organic host compounds are used to disperse the 2D perovskites, effectively creating a matrix of the dielectric quantum wells, which significantly boosts the exciton binding energy by the dielectric confinement effect. Through the Förster resonance energy transfer, the excitons down-convert and recombine radiatively in the 2D perovskites. We report room-temperature pure green (n = 7-10), sky blue (n = 5), pure blue (n = 3), and deep blue (n = 1) electroluminescence, with record-high external quantum efficiencies in the green-to-blue wavelength region.
Directory of Open Access Journals (Sweden)
Yuichi Otsuka
2016-03-01
Full Text Available The metal-insulator transition has been a subject of intense research since Mott first proposed that the metallic behavior of interacting electrons could turn to an insulating one as electron correlations increase. Here, we consider electrons with massless Dirac-like dispersion in two spatial dimensions, described by the Hubbard models on two geometrically different lattices, and perform numerically exact calculations on unprecedentedly large systems that, combined with a careful finite-size scaling analysis, allow us to explore the quantum critical behavior in the vicinity of the interaction-driven metal-insulator transition. Thereby, we find that the transition is continuous, and we determine the quantum criticality for the corresponding universality class, which is described in the continuous limit by the Gross-Neveu model, a model extensively studied in quantum field theory. Furthermore, we discuss a fluctuation-driven scenario for the metal-insulator transition in the interacting Dirac electrons: The metal-insulator transition is triggered only by the vanishing of the quasiparticle weight, not by the Dirac Fermi velocity, which instead remains finite near the transition. This important feature cannot be captured by a simple mean-field or Gutzwiller-type approximate picture but is rather consistent with the low-energy behavior of the Gross-Neveu model.
Synthesis of CdSe quantum dots for quantum dot sensitized solar cell
Energy Technology Data Exchange (ETDEWEB)
Singh, Neetu, E-mail: singh.neetu1985@gmail.com; Kapoor, Avinashi [Department of Electronic Science, University of Delhi South Campus, New Delhi-110 021 (India); Kumar, Vinod [Department of Physics, University of the Free State, Bloemfontein, ZA9300 (South Africa); Mehra, R. M. [School of Engineering and Technology, Sharda University, Greater Noida-201 306, U.P. (India)
2014-04-24
CdSe Quantum Dots (QDs) of size 0.85 nm were synthesized using chemical route. ZnO based Quantum Dot Sensitized Solar Cell (QDSSC) was fabricated using CdSe QDs as sensitizer. The Pre-synthesized QDs were found to be successfully adsorbed on front ZnO electrode and had potential to replace organic dyes in Dye Sensitized Solar Cells (DSSCs). The efficiency of QDSSC was obtained to be 2.06 % at AM 1.5.
Charged-Exciton Complexes in Quantum Dots
Institute of Scientific and Technical Information of China (English)
XIE Wen-Fang
2001-01-01
It is known experimentally that stable charged-exciton complexes can exist in low-dimensional semiconductor nanostructures. Much less is known about the properties of such charged-exciton complexes since three-body problems are very difficult to be solved, even numerically. Here we introduce the correlated hyperspherical harmonics as basis functions to solve the hyperangular equation for negatively and positively charged excitons (trions) in a harmonic quantum dot. By using this method, we have calculated the energy spectra of the low-lying states of a charged exciton as a function of the radius of quantum dot. Based on symmetry analysis, the level crossover as the dot radius increases can be fully explained as the results of symmetry constraint.``
Saturating optical resonances in quantum dots
Nair, Selvakumar V.; Rustagi, K. C.
Optical bistability in quantum dots, recently proposed by Chemla and Miller, is studied in a two-resonance model. We show that for such classical electromagnetic resonances the applicability of a two-resonance model is far more restrictive than for those in atoms.
System and method for making quantum dots
Bakr, Osman M.
2015-05-28
Embodiments of the present disclosure provide for methods of making quantum dots (QDs) (passivated or unpassivated) using a continuous flow process, systems for making QDs using a continuous flow process, and the like. In one or more embodiments, the QDs produced using embodiments of the present disclosure can be used in solar photovoltaic cells, bio-imaging, IR emitters, or LEDs.
Quantum dot waveguides: ultrafast dynamics and applications
DEFF Research Database (Denmark)
Chen, Yaohui; Mørk, Jesper
2009-01-01
In this paper we analyze, based on numerical simulations, the dynamics of semiconductor devices incorporating quantum dots (QDs). In particular we emphasize the unique ultrafast carrier dynamics occurring between discrete QD bound states, and its influence on QD semiconductor optical amplifiers...... (SOAs). Also the possibility of realizing an all-optical regenerator by incorporating a QD absorber section in an amplifier structure is discussed....
Electron Scattering in Intrananotube Quantum Dots
Buchs, G.; Bercioux, D.; Ruffieux, P.; Gröning, P.; Grabert, H.; Gröning, O.
2009-01-01
Intratube quantum dots showing particle-in-a-box-like states with level spacings up to 200 meV are realized in metallic single-walled carbon nanotubes by means of low dose medium energy Ar+ irradiation. Fourier-transform scanning tunneling spectroscopy compared to results of a Fabry-Perot electron r
Producing Quantum Dots by Spray Pyrolysis
Banger, Kulbinder; Jin, Michael H.; Hepp, Aloysius
2006-01-01
An improved process for making nanocrystallites, commonly denoted quantum dots (QDs), is based on spray pyrolysis. Unlike the process used heretofore, the improved process is amenable to mass production of either passivated or non-passivated QDs, with computer control to ensure near uniformity of size.
Enabling biomedical research with designer quantum dots
Tomczak, N.; Janczewski, D.; Dorokhin, D.V.; Han, M-Y; Vancso, G.J.; Navarro, Melba; Planell, Josep A.
2012-01-01
Quantum Dots (QDs) are a new class of semiconductor nanoparticulate luminophores, which are actively researched for novel applications in biology and nanomedicine. In this review, the recent progress in the design and applications of QD labels for in vitro and in vivo imaging of cells is presented.
Single Molecule Applications of Quantum Dots
DEFF Research Database (Denmark)
Rasmussen, Thomas Elmelund; Jauffred, Liselotte; Brewer, Jonathan R.
2013-01-01
Fluorescent nanocrystals composed of semiconductor materials were first introduced for biological applications in the late 1990s. The focus of this review is to give a brief survey of biological applications of quantum dots (QDs) at the single QD sensitivity level. These are described as follows: 1...
Spin Wigner molecules in quantum dots
Zutic, Igor; Oszwaldowski, Rafal; Stano, Peter; Petukhov, A. G.
2013-03-01
The interplay of confinement and Coulomb interactions in quantum dots can lead to strongly correlated phases differing qualitatively from the Fermi liquid behavior. While in three dimensions the correlation-induced Wigner crystal is elusive and expected only in the limit of an extremely low carrier density, its nanoscale analog, the Wigner molecule, has been observed in quantum dots at much higher densities [1]. We explore how the presence of magnetic impurities in quantum dots can provide additional opportunities to study correlation effects and the resulting ordering in carrier and impurity spins[2]. By employing exact diagonalization we reveal that seemingly simple two-carrier quantum dots lead to a rich phase diagram [2,3]. We propose experiments to verify our predictions; in particular, we discuss interband optical transitions as a function of temperature and magnetic field. DOE-BES, meta-QUTE 259 ITMS NFP Grant No. 26240120022, CE SAS QUTE, EU 260 Project Q-essence, Grant No. APVV-0646-10, and SCIEX.
Nonlinear spectroscopy of photon-dressed Dirac electrons in a quantum dot
Roslyak, O.; Gumbs, Godfrey; Mukamel, S.
2013-01-01
We study the localization of dressed Dirac electrons in a cylindrical quantum dot (QD) formed on monolayer and bilayer graphene by spatially different potential profiles. Short-lived excitonic states which are too broad to be resolved in linear spectroscopy are revealed by cross-peaks in the photon-echo nonlinear technique. Signatures of the dynamic gap in the two-dimensional photon-echo spectra are discussed.
Optical Properties of Quantum-Dot-Doped Liquid Scintillators
Aberle, C; Weiss, S; Winslow, L
2013-01-01
Semiconductor nanoparticles (quantum dots) were studied in the context of liquid scintillator development for upcoming neutrino experiments. The unique optical and chemical properties of quantum dots are particularly promising for the use in neutrinoless double beta decay experiments. Liquid scintillators for large scale neutrino detectors have to meet specific requirements which are reviewed, highlighting the peculiarities of quantum-dot-doping. In this paper, we report results on laboratory-scale measurements of the attenuation length and the fluorescence properties of three commercial quantum dot samples. The results include absorbance and emission stability measurements, improvement in transparency due to filtering of the quantum dot samples, precipitation tests to isolate the quantum dots from solution and energy transfer studies with quantum dots and the fluorophore PPO.
Optical properties of quantum-dot-doped liquid scintillators
Aberle, C.; Li, J. J.; Weiss, S.; Winslow, L.
2013-10-01
Semiconductor nanoparticles (quantum dots) were studied in the context of liquid scintillator development for upcoming neutrino experiments. The unique optical and chemical properties of quantum dots are particularly promising for the use in neutrinoless double-beta decay experiments. Liquid scintillators for large scale neutrino detectors have to meet specific requirements which are reviewed, highlighting the peculiarities of quantum-dot-doping. In this paper, we report results on laboratory-scale measurements of the attenuation length and the fluorescence properties of three commercial quantum dot samples. The results include absorbance and emission stability measurements, improvement in transparency due to filtering of the quantum dot samples, precipitation tests to isolate the quantum dots from solution and energy transfer studies with quantum dots and the fluorophore PPO.
Van Gorder, Robert A.
2016-05-01
Very recent experimental work has demonstrated the existence of Kelvin waves along quantized vortex filaments in superfluid helium. The possible configurations and motions of such filaments is of great physical interest, and Svistunov previously obtained a Hamiltonian formulation for the dynamics of quantum vortex filaments in the low-temperature limit under the assumption that the vortex filament is essentially aligned along one axis, resulting in a two-dimensional (2D) problem. It is standard to approximate the dynamics of thin filaments by employing the local induction approximation (LIA), and we show that by putting the two-dimensional LIA into correspondence with the first equation in the integrable Wadati-Konno-Ichikawa-Schimizu (WKIS) hierarchy, we immediately obtain solutions to the two-dimensional LIA, such as helix, planar, and self-similar solutions. These solutions are obtained in a rather direct manner from the WKIS equation and then mapped into the 2D-LIA framework. Furthermore, the approach can be coupled to existing inverse scattering transform results from the literature in order to obtain solitary wave solutions including the analog of the Hasimoto one-soliton for the 2D-LIA. One large benefit of the approach is that the correspondence between the 2D-LIA and the WKIS allows us to systematically obtain vortex filament solutions directly in the Cartesian coordinate frame without the need to solve back from curvature and torsion. Implications of the results for the physics of experimentally studied solitary waves, Kelvin waves, and postvortex reconnection events are mentioned.
Two-dimensional spin liquids with Z2 topological order in an array of quantum wires
Patel, Aavishkar A.; Chowdhury, Debanjan
2016-11-01
Insulating Z2 spin liquids are a phase of matter with bulk anyonic quasiparticle excitations and ground-state degeneracies on manifolds with nontrivial topology. We construct a time-reversal symmetric Z2 spin liquid in two spatial dimensions using an array of quantum wires. We identify the anyons as kinks in the appropriate Luttinger-liquid description, compute their mutual statistics, and construct local operators that transport these quasiparticles. We also present a construction of a fractionalized Fermi liquid (FL*) by coupling the spin sector of the Z2 spin liquid to a Fermi liquid via a Kondo-like coupling.
Probing the quantum-classical connection with open quantum dots
Ferry, D. K.; Akis, R.; Brunner, R.
2015-10-01
Open quantum dots provide a natural system in which to study both classical and quantum features of transport. From the classical point of view these dots possess a mixed phase space which yields families of closed, regular orbits as well as an expansive sea of chaos. As a closed test bed, they provide a natural system with a very rich set of eigen-states. When coupled to the environment through a pair of quantum point contacts, each of which passes several modes, the original quantum environment evolves into a set of decoherent and coherent states, which eventually couple to the classical states discussed above. The manner of this connection is governed strongly by decoherence theory. The remaining coherent states possess all the properties of pointer states. Here, we discuss the quantum-classical connection and how it appears within the experimental world.
Quantum Dots and Their Multimodal Applications: A Review
Directory of Open Access Journals (Sweden)
Paul H. Holloway
2010-03-01
Full Text Available Semiconducting quantum dots, whose particle sizes are in the nanometer range, have very unusual properties. The quantum dots have band gaps that depend in a complicated fashion upon a number of factors, described in the article. Processing-structure-properties-performance relationships are reviewed for compound semiconducting quantum dots. Various methods for synthesizing these quantum dots are discussed, as well as their resulting properties. Quantum states and confinement of their excitons may shift their optical absorption and emission energies. Such effects are important for tuning their luminescence stimulated by photons (photoluminescence or electric field (electroluminescence. In this article, decoupling of quantum effects on excitation and emission are described, along with the use of quantum dots as sensitizers in phosphors. In addition, we reviewed the multimodal applications of quantum dots, including in electroluminescence device, solar cell and biological imaging.
Szyniszewski, M.; Mostaani, E.; Drummond, N. D.; Fal'ko, V. I.
2017-02-01
Excitonic effects play a particularly important role in the optoelectronic behavior of two-dimensional (2D) semiconductors. To facilitate the interpretation of experimental photoabsorption and photoluminescence spectra we provide statistically exact diffusion quantum Monte Carlo binding-energy data for Mott-Wannier models of excitons, trions, and biexcitons in 2D semiconductors. We also provide contact pair densities to allow a description of contact (exchange) interactions between charge carriers using first-order perturbation theory. Our data indicate that the binding energy of a trion is generally larger than that of a biexciton in 2D semiconductors. We provide interpolation formulas giving the binding energy and contact density of 2D semiconductors as functions of the electron and hole effective masses and the in-plane polarizability.
Experimental apparatus for quantum simulation with two-dimensional 9Be + Coulomb crystals
Pyka, Karsten; Ball, Harrison; McRae, Terry; Edmunds, Claire; Lee, Michael W.; Henderson, Samuel; Biercuk, Michael J.; Quantum Control Lab Team
2015-03-01
We report on the development of a new experimental setup designed for Quantum Simulation studies at a computationally relevant scale using laser-cooled 9Be + ion-crystals in a Penning trap. The trap geometry is optimized using numerical calculations for trapping large ion crystals with enhanced optical access and reduced anharmonic perturbations. Separate loading and spectroscopy zones prevent long term drifts of the trapping parameters due to contamination of the trap electrodes with Be deposits. Our customized superconducting magnet provides a homogenous (dB/B telecom wavelength fiber laser systems in the IR via nonlinear conversion. Our new approach employs high-efficiency telecom modulators and mode-selecting cavities to generate multiple beamlines from a single Sum-frequency-Generation step. Ultimately, this newly developed setup will allow for studies of many-body spin systems with tuneable interaction strength from infinite-range to nearest-neighbour type interaction.
Two-Dimensional Dirac Fermions in a Topological Insulator: Transport in the Quantum Limit
Energy Technology Data Exchange (ETDEWEB)
Analytis, J.G.; /SIMES, Stanford /SLAC /Stanford U., Geballe Lab /Stanford U., Appl. Phys. Dept.; McDonald, R.D.; /Los Alamos; Riggs, S.C.; /Natl. High Mag. Field Lab.; Chu, J.-H.; /SIMES, Stanford /SLAC /Stanford U., Geballe Lab /Stanford U., Appl. Phys. Dept.; Boebinger, G.S.; /Natl. High Mag. Field Lab.; Fisher, I.R.; /SIMES, Stanford /SLAC /Stanford U., Geballe Lab /Stanford U., Appl. Phys. Dept.
2011-08-12
Pulsed magnetic fields of up to 55T are used to investigate the transport properties of the topological insulator Bi{sub 2}Se{sub 3} in the extreme quantum limit. For samples with a bulk carrier density of n = 2.9 x 10{sup 16} cm{sup -3}, the lowest Landau level of the bulk 3D Fermi surface is reached by a field of 4T. For fields well beyond this limit, Shubnikov-de Haas oscillations arising from quantization of the 2D surface state are observed, with the {nu} = 1 Landau level attained by a field of {approx} 35T. These measurements reveal the presence of additional oscillations which occur at fields corresponding to simple rational fractions of the integer Landau indices.
Quantum anomaly, universal relations, and breathing mode of a two-dimensional Fermi gas.
Hofmann, Johannes
2012-05-01
In this Letter, we show that the classical SO(2,1) symmetry of a harmonically trapped Fermi gas in two dimensions is broken by quantum effects. The anomalous correction to the symmetry algebra is given by a two-body operator that is well known as the contact. Taking into account this modification, we are able to derive the virial theorem for the system and a universal relation for the pressure of a homogeneous gas. The existence of an undamped breathing mode is associated with the classical symmetry. We provide an estimate for the anomalous frequency shift of this oscillation at zero temperature and compare the result with a recent experiment by [E. Vogt et al., Phys. Rev. Lett. 108, 070404 (2012)]. Discrepancies are attributed to finite temperature effects.
Shear viscosity at the Ising-nematic quantum critical point in two dimensional metals
Patel, Aavishkar A; Sachdev, Subir
2016-01-01
In a strongly interacting quantum liquid without quasiparticles, general scaling arguments imply that the dimensionless ratio $(k_B /\\hbar)\\, \\eta/s$, where $\\eta$ is the shear viscosity and $s$ is the entropy density, is a universal number. We compute the shear viscosity of the Ising-nematic critical point of metals in spatial dimension $d=2$ by an expansion below $d=5/2$. The anisotropy associated with directions parallel and normal to the Fermi surface leads to a violation of the scaling expectations: $\\eta$ scales in the same manner as a chiral conductivity, and the ratio $\\eta/s$ diverges as $T^{-2/z}$, where $z$ is the dynamic critical exponent for fermionic excitations dispersing normal to the Fermi surface.
Efficient Luminescence from Perovskite Quantum Dot Solids
Kim, Younghoon
2015-11-18
© 2015 American Chemical Society. Nanocrystals of CsPbX3 perovskites are promising materials for light-emitting optoelectronics because of their colloidal stability, optically tunable bandgap, bright photoluminescence, and excellent photoluminescence quantum yield. Despite their promise, nanocrystal-only films of CsPbX3 perovskites have not yet been fabricated; instead, highly insulating polymers have been relied upon to compensate for nanocrystals\\' unstable surfaces. We develop solution chemistry that enables single-step casting of perovskite nanocrystal films and overcomes problems in both perovskite quantum dot purification and film fabrication. Centrifugally cast films retain bright photoluminescence and achieve dense and homogeneous morphologies. The new materials offer a platform for optoelectronic applications of perovskite quantum dot solids.
Light emission from Si quantum dots
Directory of Open Access Journals (Sweden)
Philippe M. Fauchet
2005-01-01
Full Text Available Si quantum dots (QDs as small as ∼2 nm in diameter have been synthesized by a variety of techniques. Because of quantum confinement and the elimination of bulk or surface defects, these dots can emit light from the near infrared throughout the visible with quantum efficiencies in excess of 10%. The luminescence wavelength range has been extended to longer wavelengths by the addition of light-emitting rare earths such as erbium (Er. Light-emitting devices (LEDs have been fabricated and their performances are starting to approach those of direct band gap semiconductor or organic LEDs. A search for a Si QD-based laser is even under way. The state-of-the-art in the materials science, physics, and device development of luminescent Si QDs is reviewed and areas of future research are pointed out.
Quantum Size- Dependent Third- Order Nonlinear Optical Susceptibility in Semiconductor Quantum Dots
Institute of Scientific and Technical Information of China (English)
SUN Ting; XIONG Gui-guang
2005-01-01
The density matrix approach has been employed to investigate the optical nonlinear polarization in a single semiconductor quantum dot(QD). Electron states are considered to be confined within a quantum dot with infinite potential barriers. It is shown, by numerical calculation, that the third-order nonlinear optical susceptibilities for a typical Si quantum dot is dependent on the quantum size of the quantum dot and the frequency of incident light.
Local Quantum Dot Tuning on Photonic Crystal Chips
Faraon, Andrei; Fushman, Ilya; Stoltz, Nick; Petroff, Pierre; Vuckovic, Jelena
2007-01-01
Quantum networks based on InGaAs quantum dots embedded in photonic crystal devices rely on QDs being in resonance with each other and with the cavities they are embedded in. We developed a new technique based on temperature tuning to spectrally align different quantum dots located on the same chip. The technique allows for up to 1.8nm reversible on-chip quantum dot tuning.
High-resolution photoluminescence studies of single semiconductor quantum dots
DEFF Research Database (Denmark)
Leosson, Kristjan; Østergaard, John Erland; Jensen, Jacob Riis
2000-01-01
Semiconductor quantum dots, especially those formed by self-organized growth, are considered a promising material system for future optical devices [1] and the optical properties of quantum dot ensembles have been investigated in detail over the past years. Recently, considerable interest has...... developed in the study of single quantum dots, characterized by sharp atomic-like transition lines revealing their zero-dimensional density of states. Substantial information about the fundamental properties of individual quantum dots, as well as their interactions with other dots and the host lattice, can...
Sensitivity of quantum-dot semiconductor lasers to optical feedback.
O'Brien, D; Hegarty, S P; Huyet, G; Uskov, A V
2004-05-15
The sensitivity of quantum-dot semiconductor lasers to optical feedback is analyzed with a Lang-Kobayashi approach applied to a standard quantum-dot laser model. The carriers are injected into a quantum well and are captured by, or escape from, the quantum dots through either carrier-carrier or phonon-carrier interaction. Because of Pauli blocking, the capture rate into the dots depends on the carrier occupancy level in the dots. Here we show that different carrier capture dynamics lead to a strong modification of the damping of the relaxation oscillations. Regions of increased damping display reduced sensitivity to optical feedback even for a relatively large alpha factor.
Coupling of single quantum dots to a photonic crystal waveguide
DEFF Research Database (Denmark)
Lund-Hansen, Toke; Stobbe, Søren; Julsgaard, Brian
. An alternative approach is to couple the quantum dot directly to the propagating mode of a photonic waveguide. We demonstrate the coupling of single quantum dots to a photonic crystal waveguide using time-resolved spontaneous emission measurements. A pronounced effect is seen in the decay rates of dots coupled...
Electron-hole confinement symmetry in silicon quantum dots
Müller, F.; Mueller, Filipp; Konstantaras, Georgios; Spruijtenburg, P.C.; van der Wiel, Wilfred Gerard; Zwanenburg, Floris Arnoud
2015-01-01
We report electrical transport measurements on a gate-defined ambipolar quantum dot in intrinsic silicon. The ambipolarity allows its operation as either an electron or a hole quantum dot of which we change the dot occupancy by 20 charge carriers in each regime. Electron−hole confinement symmetry is
Coupling of single quantum dots to a photonic crystal waveguide
DEFF Research Database (Denmark)
Lund-Hansen, Toke; Stobbe, Søren; Julsgaard, Brian;
. An alternative approach is to couple the quantum dot directly to the propagating mode of a photonic waveguide. We demonstrate the coupling of single quantum dots to a photonic crystal waveguide using time-resolved spontaneous emission measurements. A pronounced effect is seen in the decay rates of dots coupled...
Electron-electron correlations in square-well quantum dots: direct energy minimization approach.
Goto, Hidekazu; Hirose, Kikuji
2011-04-01
Electron-electron correlations in two-dimensional square-well quantum dots are investigated using the direct energy minimization scheme. Searches for groundstate charges and spin configurations are performed with varying the sizes of dots and the number of electrons. For a two-electron system, a standout difference between the configurations with and without counting correlation energy is demonstrated. The emergence and melting of Wigner-molecule-like structures arising from the interplay between the kinetic energy and Coulombic interaction energy are described. Electron-electron correlation energies and addition energy spectra are calculated, and special electron numbers related to peculiar effects of the square well are extracted.
Xu, Cenke
Several examples of quantum spin systems and pseudo spin systems have been studied, and unconventional states of matters and phase transitions have been realized in all these systems under consideration. In the p +/- ip superconductor Josephson lattice and the p--band cold atomic system trapped in optical lattices, novel phases which behave similarly to 1+1 dimensional systems are realized, despite the fact that the real physical systems are in two or three dimensional spaces. For instance, by employing a spin-wave analysis together with a new duality transformation, we establish the existence and stability of a novel gapless "critical phase", which we refer to as a "bond algebraic liquid". This novel critical phase is analogous to the 1+1 dimensional algebraic boson liquid phase. The reason for the novel physics is that there is a quasilocal gauge symmetry in the effective low energy Hamiltonian. In a spin-1 system on the kagome lattice, and a hard-core boson system on the honeycomb lattice, the low energy physics is controlled by two components of compact U(1) gauge symmetries that emerge at low energy. Making use of the confinement nature of the 2+1 dimensional compact gauge theories and the powerful duality between gauge theories and height field theories, the crystalline phase diagrams are studied for both systems, and the transitions to other phases are also considered. These phase diagrams might be accessible in strongly correlated materials, or atomic systems in optical lattices. A novel quantum ground state of matter is realized in a bosonic model on three dimensional fcc lattice with emergent low energy excitations. The novel phase obtained is a stable gapless boson liquid phase, with algebraic boson density correlations. The stability of this phase is protected against the instanton effect and superfluidity by self-duality and large gauge symmetries on both sides of the duality. The gapless collective excitations of this phase closely resemble the
Mitigation of quantum dot cytotoxicity by microencapsulation.
Directory of Open Access Journals (Sweden)
Amelia Romoser
Full Text Available When CdSe/ZnS-polyethyleneimine (PEI quantum dots (QDs are microencapsulated in polymeric microcapsules, human fibroblasts are protected from acute cytotoxic effects. Differences in cellular morphology, uptake, and viability were assessed after treatment with either microencapsulated or unencapsulated dots. Specifically, QDs contained in microcapsules terminated with polyethylene glycol (PEG mitigate contact with and uptake by cells, thus providing a tool to retain particle luminescence for applications such as extracellular sensing and imaging. The microcapsule serves as the "first line of defense" for containing the QDs. This enables the individual QD coating to be designed primarily to enhance the function of the biosensor.
Quantum Computation Using Optically Coupled Quantum Dot Arrays
Pradhan, Prabhakar; Anantram, M. P.; Wang, K. L.; Roychowhury, V. P.; Saini, Subhash (Technical Monitor)
1998-01-01
A solid state model for quantum computation has potential advantages in terms of the ease of fabrication, characterization, and integration. The fundamental requirements for a quantum computer involve the realization of basic processing units (qubits), and a scheme for controlled switching and coupling among the qubits, which enables one to perform controlled operations on qubits. We propose a model for quantum computation based on optically coupled quantum dot arrays, which is computationally similar to the atomic model proposed by Cirac and Zoller. In this model, individual qubits are comprised of two coupled quantum dots, and an array of these basic units is placed in an optical cavity. Switching among the states of the individual units is done by controlled laser pulses via near field interaction using the NSOM technology. Controlled rotations involving two or more qubits are performed via common cavity mode photon. We have calculated critical times, including the spontaneous emission and switching times, and show that they are comparable to the best times projected for other proposed models of quantum computation. We have also shown the feasibility of accessing individual quantum dots using the NSOM technology by calculating the photon density at the tip, and estimating the power necessary to perform the basic controlled operations. We are currently in the process of estimating the decoherence times for this system; however, we have formulated initial arguments which seem to indicate that the decoherence times will be comparable, if not longer, than many other proposed models.
Coherent transport through interacting quantum dots
Energy Technology Data Exchange (ETDEWEB)
Hiltscher, Bastian
2012-10-05
The present thesis is composed of four different works. All deal with coherent transport through interacting quantum dots, which are tunnel-coupled to external leads. There a two main motivations for the use of quantum dots. First, they are an ideal device to study the influence of strong Coulomb repulsion, and second, their discrete energy levels can easily be tuned by external gate electrodes to create different transport regimes. The expression of coherence includes a very wide range of physical correlations and, therefore, the four works are basically independent of each other. Before motivating and introducing the different works in more detail, we remark that in all works a diagrammatic real-time perturbation theory is used. The fermionic degrees of freedom of the leads are traced out and the elements of the resulting reduced density matrix can be treated explicitly by means of a generalized master equation. How this equation is solved, depends on the details of the problem under consideration. In the first of the four works adiabatic pumping through an Aharonov-Bohm interferometer with a quantum dot embedded in each of the two arms is studied. In adiabatic pumping transport is generated by varying two system parameters periodically in time. We consider the two dot levels to be these two pumping parameters. Since they are located in different arms of the interferometer, pumping is a quantum mechanical effect purely relying on coherent superpositions of the dot states. It is very challenging to identify a quantum pumping mechanism in experiments, because a capacitive coupling of the gate electrodes to the leads may yield an undesired AC bias voltage, which is rectified by a time dependent conductance. Therefore, distinguishing features of these two transport mechanisms are required. We find that the dependence on the magnetic field is the key feature. While the pumped charge is an odd function of the magnetic flux, the rectified current is even, at least in
Studies of silicon quantum dots prepared at different substrate temperatures
Al-Agel, Faisal A.; Suleiman, Jamal; Khan, Shamshad A.
2017-03-01
In this research work, we have synthesized silicon quantum dots at different substrate temperatures 193, 153 and 123 K at a fixed working pressure 5 Torr. of Argon gas. The structural studies of these silicon quantum dots have been undertaken using X-ray diffraction, Field Emission Scanning Electron Microscopy (FESEM) and High Resolution Transmission Electron Microscopy (HRTEM). The optical and electrical properties have been studied using UV-visible spectroscopy, Fourier transform infrared (FTIR) spectroscopy, Fluorescence spectroscopy and I-V measurement system. X-ray diffraction pattern of Si quantum dots prepared at different temperatures show the amorphous nature except for the quantum dots synthesized at 193 K which shows polycrystalline nature. FESEM images of samples suggest that the size of quantum dots varies from 2 to 8 nm. On the basis of UV-visible spectroscopy measurements, a direct band gap has been observed for Si quantum dots. FTIR spectra suggest that as-grown Si quantum dots are partially oxidized which is due exposure of as-prepared samples to air after taking out from the chamber. PL spectra of the synthesized silicon quantum dots show an intense peak at 444 nm, which may be attributed to the formation of Si quantum dots. Temperature dependence of dc conductivity suggests that the dc conductivity enhances exponentially by raising the temperature. On the basis above properties i.e. direct band gap, high absorption coefficient and high conductivity, these silicon quantum dots will be useful for the fabrication of solar cells.
Entrapment in phospholipid vesicles quenches photoactivity of quantum dots.
Generalov, Roman; Kavaliauskiene, Simona; Westrøm, Sara; Chen, Wei; Kristensen, Solveig; Juzenas, Petras
2011-01-01
Quantum dots have emerged with great promise for biological applications as fluorescent markers for immunostaining, labels for intracellular trafficking, and photosensitizers for photodynamic therapy. However, upon entry into a cell, quantum dots are trapped and their fluorescence is quenched in endocytic vesicles such as endosomes and lysosomes. In this study, the photophysical properties of quantum dots were investigated in liposomes as an in vitro vesicle model. Entrapment of quantum dots in liposomes decreases their fluorescence lifetime and intensity. Generation of free radicals by liposomal quantum dots is inhibited compared to that of free quantum dots. Nevertheless, quantum dot fluorescence lifetime and intensity increases due to photolysis of liposomes during irradiation. In addition, protein adsorption on the quantum dot surface and the acidic environment of vesicles also lead to quenching of quantum dot fluorescence, which reappears during irradiation. In conclusion, the in vitro model of phospholipid vesicles has demonstrated that those quantum dots that are fated to be entrapped in endocytic vesicles lose their fluorescence and ability to act as photosensitizers.
Entrapment in phospholipid vesicles quenches photoactivity of quantum dots
Directory of Open Access Journals (Sweden)
Generalov R
2011-09-01
Full Text Available Roman Generalov1,2, Simona Kavaliauskiene1, Sara Westrøm1, Wei Chen3, Solveig Kristensen2, Petras Juzenas11Department of Radiation Biology, Institute for Cancer Research, Norwegian Radium Hospital, Oslo University Hospital, Oslo, Norway; 2School of Pharmacy, University of Oslo, Oslo, Norway; 3Department of Physics, The University of Texas at Arlington, Arlington, TX, USAAbstract: Quantum dots have emerged with great promise for biological applications as fluorescent markers for immunostaining, labels for intracellular trafficking, and photosensitizers for photodynamic therapy. However, upon entry into a cell, quantum dots are trapped and their fluorescence is quenched in endocytic vesicles such as endosomes and lysosomes. In this study, the photophysical properties of quantum dots were investigated in liposomes as an in vitro vesicle model. Entrapment of quantum dots in liposomes decreases their fluorescence lifetime and intensity. Generation of free radicals by liposomal quantum dots is inhibited compared to that of free quantum dots. Nevertheless, quantum dot fluorescence lifetime and intensity increases due to photolysis of liposomes during irradiation. In addition, protein adsorption on the quantum dot surface and the acidic environment of vesicles also lead to quenching of quantum dot fluorescence, which reappears during irradiation. In conclusion, the in vitro model of phospholipid vesicles has demonstrated that those quantum dots that are fated to be entrapped in endocytic vesicles lose their fluorescence and ability to act as photosensitizers.Keywords: fluorescence lifetime, free radicals, liposomes, lipodots, reactive oxygen species
Single quantum dots fundamentals, applications, and new concepts
2003-01-01
This book reviews recent advances in the exciting and rapid growing field of semiconductor quantum dots by contributions from some of the most prominent researchers in the field. Special focus is given to the optical and electronic properties of single quantum dots due to their potential applications in devices operating with single electrons and/or single photons. This includes quantum dots in electric and magnetic fields, cavity-quantum electrodynamics, nonclassical light generation, and coherent optical control of excitons. Single Quantum Dots also addresses various growth techniques as well as potential device applications such as quantum dot lasers, and new concepts like a single-photon source, and a single quantum dot laser.
Mode Competition in Dual-Mode Quantum Dots Semiconductor Microlaser
Chusseau, Laurent; Viktorovitch, P; Letartre, Xavier
2013-01-01
This paper describes the modeling of quantum dots lasers with the aim of assessing the conditions for stable cw dual-mode operation when the mode separation lies in the THz range. Several possible models suited for InAs quantum dots in InP barriers are analytically evaluated, in particular quantum dots electrically coupled through a direct exchange of excitation by the wetting layer or quantum dots optically coupled through the homogeneous broadening of their optical gain. A stable dual-mode regime is shown possible in all cases when quantum dots are used as active layer whereas a gain medium of quantum well or bulk type inevitably leads to bistable behavior. The choice of a quantum dots gain medium perfectly matched the production of dual-mode lasers devoted to THz generation by photomixing.
Peptide-Decorated Tunable-Fluorescence Graphene Quantum Dots.
Sapkota, Bedanga; Benabbas, Abdelkrim; Lin, Hao-Yu Greg; Liang, Wentao; Champion, Paul; Wanunu, Meni
2017-03-22
We report here the synthesis of graphene quantum dots with tunable size, surface chemistry, and fluorescence properties. In the size regime 15-35 nm, these quantum dots maintain strong visible light fluorescence (mean quantum yield of 0.64) and a high two-photon absorption (TPA) cross section (6500 Göppert-Mayer units). Furthermore, through noncovalent tailoring of the chemistry of these quantum dots, we obtain water-stable quantum dots. For example, quantum dots with lysine groups bind strongly to DNA in solution and inhibit polymerase-based DNA strand synthesis. Finally, by virtue of their mesoscopic size, the quantum dots exhibit good cell permeability into living epithelial cells, but they do not enter the cell nucleus.
Principles of conjugating quantum dots to proteins via carbodiimide chemistry.
Song, Fayi; Chan, Warren C W
2011-12-09
The covalent coupling of nanomaterials to bio-recognition molecules is a critical intermediate step in using nanomaterials for biology and medicine. Here we investigate the carbodiimide-mediated conjugation of fluorescent quantum dots to different proteins (e.g., immunoglobulin G, bovine serum albumin, and horseradish peroxidase). To enable these studies, we developed a simple method to isolate quantum dot bioconjugates from unconjugated quantum dots. The results show that the reactant concentrations and protein type will impact the overall number of proteins conjugated onto the surfaces of the quantum dots, homogeneity of the protein-quantum dot conjugate population, quantum efficiency, binding avidity, and enzymatic kinetics. We propose general principles that should be followed for the successful coupling of proteins to quantum dots.
SU(4) Kondo entanglement in double quantum dot devices
Bonazzola, Rodrigo; Andrade, J. A.; Facio, Jorge I.; García, D. J.; Cornaglia, Pablo S.
2017-08-01
We analyze, from a quantum information theory perspective, the possibility of realizing an SU(4) entangled Kondo regime in semiconductor double quantum dot devices. We focus our analysis on the ground-state properties and consider the general experimental situation where the coupling parameters of the two quantum dots differ. We model each quantum dot with an Anderson-type Hamiltonian including an interdot Coulomb repulsion and tunnel couplings for each quantum dot to independent fermionic baths. We find that the spin and pseudospin entanglements can be made equal, and the SU(4) symmetry recovered, if the gate voltages are chosen in such a way that the average charge occupancies of the two quantum dots are equal, and the double occupancy on the double quantum dot is suppressed. We present density matrix renormalization group numerical results for the spin and pseudospin entanglement entropies, and analytical results for a simplified model that captures the main physics of the problem.
Probing relaxation times in graphene quantum dots
Volk, Christian; Neumann, Christoph; Kazarski, Sebastian; Fringes, Stefan; Engels, Stephan; Haupt, Federica; Müller, André; Stampfer, Christoph
2013-01-01
Graphene quantum dots are attractive candidates for solid-state quantum bits. In fact, the predicted weak spin-orbit and hyperfine interaction promise spin qubits with long coherence times. Graphene quantum dots have been extensively investigated with respect to their excitation spectrum, spin-filling sequence and electron-hole crossover. However, their relaxation dynamics remain largely unexplored. This is mainly due to challenges in device fabrication, in particular concerning the control of carrier confinement and the tunability of the tunnelling barriers, both crucial to experimentally investigate decoherence times. Here we report pulsed-gate transient current spectroscopy and relaxation time measurements of excited states in graphene quantum dots. This is achieved by an advanced device design that allows to individually tune the tunnelling barriers down to the low megahertz regime, while monitoring their asymmetry. Measuring transient currents through electronic excited states, we estimate a lower bound for charge relaxation times on the order of 60–100 ns. PMID:23612294
High-field studies of quantum oscillations in quasi-two-dimensional organic metals
Sandhu, Pravindrajit
frequencies in the dHvA signal is found to be a quantum mechanical effect arising from differences in field dependence of the states in the two partially occupied bands near the Fermi level.
Reconfigurable quadruple quantum dots in a silicon nanowire transistor
Energy Technology Data Exchange (ETDEWEB)
Betz, A. C., E-mail: ab2106@cam.ac.uk; Broström, M.; Gonzalez-Zalba, M. F. [Hitachi Cambridge Laboratory, J. J. Thomson Avenue, Cambridge CB3 0HE (United Kingdom); Tagliaferri, M. L. V. [Laboratorio MDM, CNR-IMM, Via C. Olivetti 2, 20864 Agrate Brianza (MB) (Italy); Dipartimento di Scienza dei Materiali, Universit di Milano-Bicocca, Via Cozzi 53, 20125 Milano (Italy); Vinet, M. [CEA/LETI-MINATEC, CEA-Grenoble, 17 rue des martyrs, F-38054 Grenoble (France); Sanquer, M. [SPSMS, UMR-E CEA/UJF-Grenoble 1, INAC, 17 rue des Martyrs, 38054 Grenoble (France); Ferguson, A. J. [Cavendish Laboratory, University of Cambridge, Cambridge CB3 0HE (United Kingdom)
2016-05-16
We present a reconfigurable metal-oxide-semiconductor multi-gate transistor that can host a quadruple quantum dot in silicon. The device consists of an industrial quadruple-gate silicon nanowire field-effect transistor. Exploiting the corner effect, we study the versatility of the structure in the single quantum dot and the serial double quantum dot regimes and extract the relevant capacitance parameters. We address the fabrication variability of the quadruple-gate approach which, paired with improved silicon fabrication techniques, makes the corner state quantum dot approach a promising candidate for a scalable quantum information architecture.
Effect of the Electron-Phonon Coupling on Barrier D- Quantum Dots in Magnetic Fields
Institute of Scientific and Technical Information of China (English)
XIE Wen-Fang
2002-01-01
The influence of the electron-phonon coupling on the energy of low-lying states of the barrier D- center,which consists of a positive ion located on the z-axis at a distance from the two-dimensional quantum dot plane and two electrons in the dot plane bound by the ion, is investigated at arbitrary strength of magnetic field by making use of the method of few-body physics. Discontinuous ground-state energy transitions induced by the magnetic field are reported.The dependence of the binding energy of the D- ground state on the quantum dot radius is obtained. A considerable enhancement of the binding is found for the D- ground state, which results from the confinement of electrons and electron-phonon coupling.
Irie, Hiroshi; Todt, Clemens; Kumada, Norio; Harada, Yuichi; Sugiyama, Hiroki; Akazaki, Tatsushi; Muraki, Koji
2016-10-01
We study coherent transport and bound state formation of Bogoliubov quasiparticles in a high-mobility I n0.75G a0.25As two-dimensional electron gas (2DEG) coupled to a superconducting Nb electrode by means of a quantum point contact (QPC) as a tunable single-mode probe. Below the superconducting critical temperature of Nb, the QPC shows a single-channel conductance greater than the conductance quantum 2 e2/h at zero bias, which indicates the presence of Andreev-reflected quasiparticles, time-reversed states of the injected electron, returning back through the QPC. The marked sensitivity of the conductance enhancement to voltage bias and perpendicular magnetic field suggests a mechanism analogous to reflectionless tunneling—a hallmark of phase-coherent transport, with the boundary of the 2DEG cavity playing the role of scatterers. When the QPC transmission is reduced to the tunneling regime, the differential conductance vs bias voltage probes the single-particle density of states in the proximity area. Measured conductance spectra show a double peak within the superconducting gap of Nb, demonstrating the formation of Andreev bound states in the 2DEG. Both of these results, obtained in the open and closed geometries, underpin the coherent nature of quasiparticles, i.e., phase-coherent Andreev reflection at the InGaAs/Nb interface and coherent propagation in the ballistic 2DEG.
Tollerud, Jonathan O
2016-01-01
We identify carrier scattering at densities below which it has previously been observed in semiconductor quantum wells. These effects are evident in the peakshapes of 2D double-quantum spectra, which change as a function of excitation density. At high excitation densities ($\\geq 10^{9}$ carriers/,cm$^{-2}$) we observe untilted peaks similar to those reported in previous experiments. At low excitation densities (<$10^{8}$ carriers cm$^{-2}$) we observe narrower, tilted peaks. Using a simple simulation, we show that tilted peak-shapes are expected in double-quantum spectra when inhomogeneous broadening is much larger than homogeneous broadening, and that fast pure-decoherence of the double-quantum coherence can obscure this peak tilt. These results show that carrier interactions are important at lower densities than previously expected, and that the `natural' double-quantum peakshapes are hidden by carrier interactions at the excitation densities typically used. Furthermore, these results demonstrate that an...
Britton, Joseph W; Sawyer, Brian C; Keith, Adam C; Wang, C-C Joseph; Freericks, James K; Uys, Hermann; Biercuk, Michael J; Bollinger, John J
2012-04-25
The presence of long-range quantum spin correlations underlies a variety of physical phenomena in condensed-matter systems, potentially including high-temperature superconductivity. However, many properties of exotic, strongly correlated spin systems, such as spin liquids, have proved difficult to study, in part because calculations involving N-body entanglement become intractable for as few as N ≈ 30 particles. Feynman predicted that a quantum simulator--a special-purpose 'analogue' processor built using quantum bits (qubits)--would be inherently suited to solving such problems. In the context of quantum magnetism, a number of experiments have demonstrated the feasibility of this approach, but simulations allowing controlled, tunable interactions between spins localized on two- or three-dimensional lattices of more than a few tens of qubits have yet to be demonstrated, in part because of the technical challenge of realizing large-scale qubit arrays. Here we demonstrate a variable-range Ising-type spin-spin interaction, J(i,j), on a naturally occurring, two-dimensional triangular crystal lattice of hundreds of spin-half particles (beryllium ions stored in a Penning trap). This is a computationally relevant scale more than an order of magnitude larger than previous experiments. We show that a spin-dependent optical dipole force can produce an antiferromagnetic interaction J(i,j) proportional variant d(-a)(i,j), where 0 ≤ a ≤ 3 and d(i,j) is the distance between spin pairs. These power laws correspond physically to infinite-range (a = 0), Coulomb-like (a = 1), monopole-dipole (a = 2) and dipole-dipole (a = 3) couplings. Experimentally, we demonstrate excellent agreement with a theory for 0.05 ≲ a ≲ 1.4. This demonstration, coupled with the high spin count, excellent quantum control and low technical complexity of the Penning trap, brings within reach the simulation of otherwise computationally intractable problems in quantum magnetism.
Quantum Entanglement of Quantum Dot Spin Using Flying Qubits
2015-05-01
SPDC photon is teleported to a single quantum dot spin by a projective measurement using a Hong Ou Mandel (HOM) interferometer. The SPDC source...photo diode B: Blue CW: Continuous wave DBR: Distributed Bragg reflector EOM: Electro-optics modulator H: Horizontal HOM: Hong-Ou- Mandel InAs
Quantum optics with quantum dots in photonic wires
DEFF Research Database (Denmark)
Munsch, Mathieu; Cadeddu, Davide; Teissier, Jean
2016-01-01
We present an exploration of the spectroscopy of a single quantum dot in a photonic wire. The device presents a high photon extraction efficiency, and strong hybrid coupling to mechanical modes. We use resonance fluorescence to probe the emitter's properties with the highest sensitivity, allowing...
Quantum photonics with quantum dots in photonic wires
DEFF Research Database (Denmark)
Munsch, Mathieu; Kuhlmann, Andreas; Cadeddu, Davide;
2016-01-01
We present results from the spectroscopy of a single quantum dot in a photonic wire. The device presents a high photon extraction efficiency, and strong hybrid coupling to mechanical modes. We use resonance fluorescence to probe the emitter’s properties with the highest sensitivity. Weperform...
Bianucci, Pablo
Modern communications technology has encouraged an intimate connection between Semiconductor Physics and Optics, and this connection shows best in the combination of electron-confining structures with light-confining structures. Semiconductor quantum dots are systems engineered to trap electrons in a mesoscopic scale (the are composed of ≈ 10000 atoms), resulting in a behavior resembling that of atoms, but much richer. Optical microresonators are engineered to confine light, increasing its intensity and enabling a much stronger interaction with matter. Their combination opens a myriad of new directions, both in fundamental Physics and in possible applications. This dissertation explores both semiconductor quantum dots and microresonators, through experimental work done with semiconductor quantum dots and microsphere resonators spanning the fields of Quantum Optics, Quantum Information and Photonics; from quantum algorithms to polarization converters. Quantum Optics leads the way, allowing us to understand how to manipulate and measure quantum dots with light and to elucidate the interactions between them and microresonators. In the Quantum Information area, we present a detailed study of the feasibility of excitons in quantum dots to perform quantum computations, including an experimental demonstration of the single-qubit Deutsch-Jozsa algorithm performedin a single semiconductor quantum dot. Our studies in Photonics involve applications of microsphere resonators, which we have learned to fabricate and characterize. We present an elaborate description of the experimental techniques needed to study microspheres, including studies and proof of concept experiments on both ultra-sensitive microsphere sensors and whispering gallery mode polarization converters.
Nanobeam photonic crystal cavity quantum dot laser
Gong, Yiyang; Shambat, Gary; Sarmiento, Tomas; Harris, James S; Vuckovic, Jelena
2010-01-01
The lasing behavior of one dimensional GaAs nanobeam cavities with embedded InAs quantum dots is studied at room temperature. Lasing is observed throughout the quantum dot PL spectrum, and the wavelength dependence of the threshold is calculated. We study the cavity lasers under both 780 nm and 980 nm pump, finding thresholds as low as 0.3 uW and 19 uW for the two pump wavelengths, respectively. Finally, the nanobeam cavity laser wavelengths are tuned by up to 7 nm by employing a fiber taper in near proximity to the cavities. The fiber taper is used both to efficiently pump the cavity and collect the cavity emission.
Energy level statistics of quantum dots.
Tsau, Chien-Yu; Nghiem, Diu; Joynt, Robert; Woods Halley, J
2007-05-08
We investigate the charging energy level statistics of disordered interacting electrons in quantum dots by numerical calculations using the Hartree approximation. The aim is to obtain a global picture of the statistics as a function of disorder and interaction strengths. We find Poisson statistics at very strong disorder, Wigner-Dyson statistics for weak disorder and interactions, and a Gaussian intermediate regime. These regimes are as expected from previous studies and fundamental considerations, but we also find interesting and rather broad crossover regimes. In particular, intermediate between the Gaussian and Poisson regimes we find a two-sided exponential distribution for the energy level spacings. In comparing with experiment, we find that this distribution may be realized in some quantum dots.
Many electron effects in semiconductor quantum dots
Indian Academy of Sciences (India)
R K Pandey; Manoj K Harbola; V Ranjan; Vijay A Singh
2003-01-01
Semiconductor quantum dots (QDs) exhibit shell structures, very similar to atoms. Termed as ‘artificial atoms’ by some, they are much larger (1 100 nm) than real atoms. One can study a variety of manyelectron effects in them, which are otherwise difficult to observe in a real atom. We have treated these effects within the local density approximation (LDA) and the Harbola–Sahni (HS) scheme. HS is free of the selfinteraction error of the LDA. Our calculations have been performed in a three-dimensional quantum dot. We have carried out a study of the size and shape dependence of the level spacing. Scaling laws for the Hubbard ‘’ are established.
Energy level statistics of quantum dots
Energy Technology Data Exchange (ETDEWEB)
Tsau, C-Y [University of Wisconsin-Madison, Madison, WI 53706 (United States); Nghiem, Diu [University of Wisconsin-Madison, Madison, WI 53706 (United States); Joynt, Robert [University of Wisconsin-Madison, Madison, WI 53706 (United States); Halley, J Woods [School of Physics and Astronomy, University of Minnesota, Minneapolis, MN 55455 (United States)
2007-05-08
We investigate the charging energy level statistics of disordered interacting electrons in quantum dots by numerical calculations using the Hartree approximation. The aim is to obtain a global picture of the statistics as a function of disorder and interaction strengths. We find Poisson statistics at very strong disorder, Wigner-Dyson statistics for weak disorder and interactions, and a Gaussian intermediate regime. These regimes are as expected from previous studies and fundamental considerations, but we also find interesting and rather broad crossover regimes. In particular, intermediate between the Gaussian and Poisson regimes we find a two-sided exponential distribution for the energy level spacings. In comparing with experiment, we find that this distribution may be realized in some quantum dots.
Energy level statistics of quantum dots
Tsau, Chien-Yu; Nghiem, Diu; Joynt, Robert; Halley, J. Woods
2007-05-01
We investigate the charging energy level statistics of disordered interacting electrons in quantum dots by numerical calculations using the Hartree approximation. The aim is to obtain a global picture of the statistics as a function of disorder and interaction strengths. We find Poisson statistics at very strong disorder, Wigner-Dyson statistics for weak disorder and interactions, and a Gaussian intermediate regime. These regimes are as expected from previous studies and fundamental considerations, but we also find interesting and rather broad crossover regimes. In particular, intermediate between the Gaussian and Poisson regimes we find a two-sided exponential distribution for the energy level spacings. In comparing with experiment, we find that this distribution may be realized in some quantum dots.
Vacuum Rabi splitting with a single quantum dot in a photonic crystal nanocavity
Yoshie, T.; Scherer, A.; Hendrickson, J.; Khitrova, G.; Gibbs, H. M.; Rupper, G.; Ell, C.; Shchekin, O. B.; Deppe, D. G.
2004-11-01
Cavity quantum electrodynamics (QED) systems allow the study of a variety of fundamental quantum-optics phenomena, such as entanglement, quantum decoherence and the quantum-classical boundary. Such systems also provide test beds for quantum information science. Nearly all strongly coupled cavity QED experiments have used a single atom in a high-quality-factor (high-Q) cavity. Here we report the experimental realization of a strongly coupled system in the solid state: a single quantum dot embedded in the spacer of a nanocavity, showing vacuum-field Rabi splitting exceeding the decoherence linewidths of both the nanocavity and the quantum dot. This requires a small-volume cavity and an atomic-like two-level system. The photonic crystal slab nanocavity-which traps photons when a defect is introduced inside the two-dimensional photonic bandgap by leaving out one or more holes-has both high Q and small modal volume V, as required for strong light-matter interactions. The quantum dot has two discrete energy levels with a transition dipole moment much larger than that of an atom, and it is fixed in the nanocavity during growth.
Quantum dot behavior in transition metal dichalcogenides nanostructures
Luo, Gang; Zhang, Zhuo-Zhi; Li, Hai-Ou; Song, Xiang-Xiang; Deng, Guang-Wei; Cao, Gang; Xiao, Ming; Guo, Guo-Ping
2017-08-01
Recently, transition metal dichalcogenides (TMDCs) semiconductors have been utilized for investigating quantum phenomena because of their unique band structures and novel electronic properties. In a quantum dot (QD), electrons are confined in all lateral dimensions, offering the possibility for detailed investigation and controlled manipulation of individual quantum systems. Beyond the definition of graphene QDs by opening an energy gap in nanoconstrictions, with the presence of a bandgap, gate-defined QDs can be achieved on TMDCs semiconductors. In this paper, we review the confinement and transport of QDs in TMDCs nanostructures. The fabrication techniques for demonstrating two-dimensional (2D) materials nanostructures such as field-effect transistors and QDs, mainly based on e-beam lithography and transfer assembly techniques are discussed. Subsequently, we focus on electron transport through TMDCs nanostructures and QDs. With steady improvement in nanoscale materials characterization and using graphene as a springboard, 2D materials offer a platform that allows creation of heterostructure QDs integrated with a variety of crystals, each of which has entirely unique physical properties.
Research Progress of Photoanodes for Quantum Dot Sensitized Solar Cells
Directory of Open Access Journals (Sweden)
LI Zhi-min
2017-08-01
Full Text Available This paper presents the development status and tendency of quantum dot sensitized solar cells. Photoanode research progress and its related technologies are analyzed in detail from the three ways of semiconductor thin films, quantum dot co-sensitization and quantum dot doping, deriving from the approach that the conversion efficiency can be improved by photoanode modification for quantum dot sensitized solar cells. According to the key factors which restrict the cell efficiency, the promising future development of quantum dot sensitized solar cells is proposed,for example,optimizing further the compositions and structures of semiconductor thin films for the photoanodes, exploring new quantum dots with broadband absorption and developing high efficient techniques of interface modification.
DLTS measurements on GaSb/GaAs quantum dots
Energy Technology Data Exchange (ETDEWEB)
Hoegner, Annika; Nowozin, Tobias; Marent, Andreas; Bimberg, Dieter [Institut fuer Festkoerperphysik, TU Berlin (Germany); Tseng, Chi-Che [Institute of Photonics Technologies, NTHU (China); Lin, Shih-Yen [Institute of Optoelectronic Sciences, NTOU (China)
2010-07-01
Memory devices based on hole storage in self-organized quantum dots offer significant advantages with respect to storage time and scalability. Recently, we demonstrated a first prototype based on InAs/GaAs quantum dots at low temperatures. To enable feasible storage times at room temperature the localisation energy of the quantum dots has to be increased by using other material systems. A first step in this direction is the use of GaSb quantum dots within a GaAs matrix. We have characterized self-organized GaSb/GaAs quantum dots embedded into a n{sup +}p-diode structure. DLTS measurements on hole emission were conducted and yield a strong peak from which a mean emission energy of about 400 meV can be extracted. The reference sample without the quantum dots (containing only the wetting layer) shows no such peak.
Electric and Magnetic Interaction between Quantum Dots and Light
DEFF Research Database (Denmark)
Tighineanu, Petru
a future challenge for the droplet-epitaxy technique. A multipolar theory of spontaneous emission from quantum dots is developed to explain the recent observation that In(Ga)As quantum dots break the dipole theory. The analysis yields a large mesoscopic moment, which contains magnetic-dipole and electric......-matter interaction of both electric and magnetic character. Our study demonstrates that In(Ga)As quantum dots lack parity symmetry and, as consequence, can be employed for locally probing the parity symmetry of complex photonic nanostructures. This opens the prospect for interfacing quantum dots with optical......The present thesis reports research on the optical properties of quantum dots by developing new theories and conducting optical measurements. We demonstrate experimentally singlephoton superradiance in interface-uctuation quantum dots by recording the temporal decay dynamics in conjunction...
Quantum dot spectroscopy using a single phosphorus donor
Büch, Holger; Fuechsle, Martin; Baker, William; House, Matthew G.; Simmons, Michelle Y.
2015-12-01
Using a deterministic single P donor placed with atomic precision accuracy next to a nanoscale silicon quantum dot, we present a way to analyze the energy spectrum of small quantum dots in silicon by tunnel-coupled transport measurements. The energy-level structure of the quantum dot is observed as resonance features within the transport bias triangles when the donor chemical potential is aligned with states within the quantum dot as confirmed by a numeric rate equation solver SIMON. This technique allows us to independently extract the quantum dot level structure irrespective of the density of states in the leads. Such a method is useful for the investigation of silicon quantum dots in the few-electron regime where the level structure is governed by an intricate interplay between the spin- and the valley-orbit degrees of freedom.
Decoherence in Nearly-Isolated Quantum Dots
DEFF Research Database (Denmark)
Folk, J.; M. Marcus, C.; Harris jr, J.
2000-01-01
Decoherence in nearly-isolated GaAs quantum dots is investigated using the change in average Coulomb blockade peak height upon breaking time-reversal symmetry. The normalized change in average peak height approaches the predicted universal value of 1/4 at temperatures well below the single......-particle level spacing, but is greatly suppressed for temperature greater than the level spacing, suggesting that inelastic scattering or other dephasing mechanisms dominate in this regime....
Quantum-dot excitons in nanostructured environments
DEFF Research Database (Denmark)
Hvam, Jørn Märcher; Stobbe, Søren; Lodahl, Peter
2011-01-01
The interaction between light and quantum-dot (QD) excitons is strongly influenced by the environment in which the QD is placed. We have investigated the interaction by measuring the time-resolved spontaneous-emission rate of QD excitons in different nanostructured environments. Thereby, we have...... is demonstrated and the influence of disorder is discussed. The findings have a strong bearing on future nanophotonic devices....
Quantum-dot excitons in nanostructured environments
DEFF Research Database (Denmark)
Hvam, Jørn Märcher; Stobbe, Søren; Lodahl, Peter
2010-01-01
The interaction between light and quantum-dot (QD) excitons is strongly influenced by the environment in which the QD is placed. We have investigated the interaction by measuring the time-resolved spontaneous-emission rate of QD excitons in different nanostructured environments. Thereby, we have...... is demonstrated and the influence of disorder is discussed. The findings have a strong bearing on future nanophotonic devices....
Quantum dot/glycol chitosan fluorescent nanoconjugates
Mansur, Alexandra AP; Herman S. Mansur
2015-01-01
In this study, novel carbohydrate-based nanoconjugates combining chemically modified chitosan with semiconductor quantum dots (QDs) were designed and synthesised via single-step aqueous route at room temperature. Glycol chitosan (G-CHI) was used as the capping ligand aiming to improve the water solubility of the nanoconjugates to produce stable and biocompatible colloidal systems. UV-visible (UV–vis) spectroscopy, photoluminescence (PL) spectroscopy, and Fourier transform infrared (FTIR) spec...
Depleted bulk heterojunction colloidal quantum dot photovoltaics
Energy Technology Data Exchange (ETDEWEB)
Barkhouse, D.A.R. [Department of Electrical and Computer Engineering, University of Toronto, 10 King' s College Road, Toronto, Ontario M5S 3G4 (Canada); IBM Thomas J. Watson Research Center, Kitchawan Road, Yorktown Heights, NY, 10598 (United States); Debnath, Ratan; Kramer, Illan J.; Zhitomirsky, David; Levina, Larissa; Sargent, Edward H. [Department of Electrical and Computer Engineering, University of Toronto, 10 King' s College Road, Toronto, Ontario M5S 3G4 (Canada); Pattantyus-Abraham, Andras G. [Department of Electrical and Computer Engineering, University of Toronto, 10 King' s College Road, Toronto, Ontario M5S 3G4 (Canada); Quantum Solar Power Corporation, 1055 W. Hastings, Ste. 300, Vancouver, BC, V6E 2E9 (Canada); Etgar, Lioz; Graetzel, Michael [Laboratory for Photonics and Interfaces, Institute of Chemical Sciences and Engineering, School of Basic Sciences, Swiss Federal Institute of Technology, CH-1015 Lausanne (Switzerland)
2011-07-26
The first solution-processed depleted bulk heterojunction colloidal quantum dot solar cells are presented. The architecture allows for high absorption with full depletion, thereby breaking the photon absorption/carrier extraction compromise inherent in planar devices. A record power conversion of 5.5% under simulated AM 1.5 illumination conditions is reported. (Copyright copyright 2011 WILEY-VCH Verlag GmbH and Co. KGaA, Weinheim)
The Silicon:Colloidal Quantum Dot Heterojunction
Masala, Silvia
2015-10-13
A heterojunction between crystalline silicon and colloidal quantum dots (CQDs) is realized. A special interface modification is developed to overcome an inherent energetic band mismatch between the two semiconductors, and realize the efficient collection of infrared photocarriers generated in the CQD film. This junction is used to produce a sensitive near infrared photodetector. © 2015 WILEY-VCH Verlag GmbH & Co. KGaA, Weinheim.
Depleted Bulk Heterojunction Colloidal Quantum Dot Photovoltaics
Barkhouse, D. Aaron R.
2011-05-26
The first solution-processed depleted bulk heterojunction colloidal quantum dot solar cells are presented. The architecture allows for high absorption with full depletion, thereby breaking the photon absorption/carrier extraction compromise inherent in planar devices. A record power conversion of 5.5% under simulated AM 1.5 illumination conditions is reported. Copyright © 2011 WILEY-VCH Verlag GmbH & Co. KGaA, Weinheim.
Pharmaceutical and biomedical applications of quantum dots.
Bajwa, Neha; Mehra, Neelesh K; Jain, Keerti; Jain, Narendra K
2016-05-01
Quantum dots (QDs) have captured the fascination and attention of scientists due to their simultaneous targeting and imaging potential in drug delivery, in pharmaceutical and biomedical applications. In the present study, we have exhaustively reviewed various aspects of QDs, highlighting their pharmaceutical and biomedical applications, pharmacology, interactions, and toxicological manifestations. The eventual use of QDs is to dramatically improve clinical diagnostic tests for early detection of cancer. In recent years, QDs were introduced to cell biology as an alternative fluorescent probe.
The pinning effect in quantum dots
Energy Technology Data Exchange (ETDEWEB)
Monisha, P. J., E-mail: pjmonisha@gmail.com [School of Physics, University of Hyderabad, Hyderabad-500046 (India); Mukhopadhyay, Soma [Department of Physics, D V R College of Engineering and Technology, Hyderabad-502285 (India)
2014-04-24
The pinning effect is studied in a Gaussian quantum dot using the improved Wigner-Brillouin perturbation theory (IWBPT) in the presence of electron-phonon interaction. The electron ground state plus one phonon state is degenerate with the electron in the first excited state. The electron-phonon interaction lifts the degeneracy and the first excited states get pinned to the ground state plus one phonon state as we increase the confinement frequency.
Electrically addressing a single self-assembled quantum dot
Ellis, D J P; Atkinson, P; Ritchie, D A; Shields, A J
2006-01-01
We report on the use of an aperture in an aluminum oxide layer to restrict current injection into a single self-assembled InAs quantum dot, from an ensemble of such dots within a large mesa. The insulating aperture is formed through the wet-oxidation of a layer of AlAs. Under photoluminescence we observe that only one quantum dot in the ensemble exhibits a Stark shift, and that the same single dot is visible under electroluminescence. Autocorrelation measurements performed on the electroluminescence confirm that we are observing emission from a single quantum dot.
Electron States of Few-Electron Quantum Dots
Institute of Scientific and Technical Information of China (English)
戴振宏; 孙金祚; 张立德; 李作宏; 黄士勇; 隋鹏飞
2002-01-01
We study few-electron semiconductor quantum dots using the unrestricted Hartree-Fock-Roothaan method based on the Gaussian basis. Our emphasis is on the energy level calculation for quantum dots. The confinement potential in a quantum dot is assumed to be in a form of three-dimensional spherical finite potential well. Some valuable results, such as the rearrangement of the energy level, have been obtained.
Semiconductor quantum dot scintillation under gamma-ray irradiation.
Létant, S E; Wang, T-F
2006-12-01
We recently demonstrated the ability of semiconductor quantum dots to convert alpha radiation into visible photons. In this letter, we report on the scintillation of quantum dots under gamma irradiation and compare the energy resolution of the 59 keV line of americium-241 obtained with our quantum dot-glass nanocomposite to that of a standard sodium iodide scintillator. A factor 2 improvement is demonstrated experimentally and interpreted theoretically using a combination of energy-loss and photon-transport models.
Controllability of multi-partite quantum systems and selective excitation of quantum dots
Energy Technology Data Exchange (ETDEWEB)
Schirmer, S G [Department of Applied Mathematics and Theoretical Physics, University of Cambridge, Wilberforce Road, Cambridge CB3 0WA (United Kingdom); Pullen, I C H [Department of Applied Mathematics and Computing, Open University, Walton Hall, Milton Keynes MK7 6AA (United Kingdom); Solomon, A I [Department of Physics and Astronomy, Open University, Walton Hall, Milton Keynes MK7 6AA (United Kingdom)
2005-10-01
We consider the degrees of controllability of multi-partite quantum systems, as well as necessary and sufficient criteria for each case. The results are applied to the problem of simultaneous control of an ensemble of quantum dots with a single laser pulse. Finally, we apply optimal control techniques to demonstrate selective excitation of individual dots for a simultaneously controllable ensemble of quantum dots.
Quantum optics with quantum dots in photonic nanowires
DEFF Research Database (Denmark)
Claudon, Julien; Munsch, Matthieu; Bleuse, Joel;
2012-01-01
Besides microcavities and photonic crystals, photonic nanowires have recently emerged as a novel resource for solidstate quantum optics. We will review recent studies which demonstrate an excellent control over the spontaneous emission of InAs quantum dots (QDs) embedded in single-mode Ga...... quantum optoelectronic devices. Quite amazingly, this approach has for instance permitted (unlike microcavity-based approaches) to combine for the first time a record-high efficiency (72%) and a negligible g(2) in a QD single photon source....
Quantum transport through an array of quantum dots.
Chen, Shuguang; Xie, Hang; Zhang, Yu; Cui, Xiaodong; Chen, Guanhua
2013-01-07
The transient current through an array of as many as 1000 quantum dots is simulated with two newly developed quantum mechanical methods. To our surprise, upon switching on the bias voltage, the current increases linearly with time before reaching its steady state value. And the time required for the current to reach its steady state value is proportional to the length of the array, and more interestingly, is exactly the time for a conducting electron to travel through the array at the Fermi velocity. These quantum phenomena can be understood by a simple analysis on the energetics of an equivalent classical circuit. An experimental design is proposed to confirm the numerical findings.
Tuning the quantum critical crossover in quantum dots
Murthy, Ganpathy
2005-03-01
Quantum dots with large Thouless number g embody a regime where both disorder and interactions can be treated nonperturbatively using large-N techniques (with N=g) and quantum phase transitions can be studied. Here we focus on dots where the noninteracting Hamiltonian is drawn from a crossover ensemble between two symmetry classes, where the crossover parameter introduces a new, tunable energy scale independent of and much smaller than the Thouless energy. We show that the quantum critical regime, dominated by collective critical fluctuations, can be accessed at the new energy scale. The nonperturbative physics of this regime can only be described by the large-N approach, as we illustrate with two experimentally relevant examples. G. Murthy, PRB 70, 153304 (2004). G. Murthy, R. Shankar, D. Herman, and H. Mathur, PRB 69, 075321 (2004)
Investigation of Quantum Dot Lasers
2007-11-02
Lett. 79, 722 (2001). 8. Report of Inventions None. 9. List of Scientific Personnel Supported, Degrees, Awards and Honors Siddhartha ...Ghosh, GSRA Sameer Pradhan, GSRA Sasan Fathpour, GSRA Zetian Mi, GSRA Siddhartha Ghosh, Ph.D., “Growth of In(Ga)As/GaAs self-organized quantum
Elafandy, Rami T.
2011-12-01
Comparison between indium rich (27%) InGaN/GaN quantum dots (QDs) and their underlying wetting layer (WL) is performed by means of optical and structural characterizations. With increasing temperature, micro-photoluminescence (μPL) study reveals the superior ability of QDs to prevent carrier thermalization to nearby traps compared to the two dimensional WL. Thus, explaining the higher internal quantum efficiency of the QD nanostructure compared to the higher dimensional WL. Structural characterization (X-ray diffraction (XRD)) and transmission electron microscopy (TEM)) reveal an increase in the QD indium content over the WL indium content which is due to strain induced drifts. © 2011 IEEE.
Li, Xiaoqiang; Wang, Peng; Xu, Zhijuan; Zhong, Huikai; Wu, Zhiqian; Lin, Shisheng
2015-01-01
Photo-induced doping is employed into graphene based solar cell through designing of a novel type of solar cell based on graphene/CdTe Schottky heterostructure. By coating a layer of ultrathin CdSe quantum dots onto graphene/CdTe heterostructure, the performance of the graphene/CdTe solar cell is improved by about 50%. Photo-induced doping is mainly accounted for this enhancement, as evidenced by resistance, photoluminescence and quantum efficiency measurements. This work demonstrates a general and feasible way of designing novel type of solar cells based on two dimensional materials/semiconductor heterostructures.
Directory of Open Access Journals (Sweden)
Isnaeni Isnaeni
2016-09-01
Full Text Available Two-dimensional photonic crystal structures not only confine light and guide waves laterally but also reflect light in the normal direction due to a slow Bloch mode effect. However, evidence of the utilization of this structure as a mirror is required. Therefore, in this work, a simulation was made and experimental results were obtained to prove that there was an increase in the intensity of reflected CdSe colloidal quantum dots emission in the normal direction when a 2D photonic crystal structure was used. A thin TiO2 film was shaped into a two-dimensional photonic crystal structure using a simple sol-gel and polystyrene-mask-etching procedure. This structure was then placed on top of the thin CdSe quantum dots film layer. The emission of quantum dots onto the two-dimensional photonic crystal structure was compared to quantum dots emission onto a flat, thin TiO2 film. An increase in the quantum dots emission of up to 105% was in the presence of the two-dimensional photonic crystal structure. This finding is very useful for photonic device applications, such as light-emitting diodes, laser systems and bio-tagging detection systems.
Polarized quantum dot emission in electrohydrodynamic jet printed photonic crystals
Energy Technology Data Exchange (ETDEWEB)
See, Gloria G. [Micro and Nanotechnology Laboratory, Department of Electrical and Computer Engineering, University of Illinois at Urbana-Champaign, 208 North Wright Street, Urbana, Illinois 61801 (United States); Xu, Lu; Nuzzo, Ralph G. [Department of Chemistry, University of Illinois at Urbana-Champaign, 600 South Mathews Avenue, Urbana, Illinois 61801 (United States); Sutanto, Erick; Alleyne, Andrew G. [Mechanical Science and Engineering Department, University of Illinois at Urbana-Champaign, 154 Mechanical Engineering Building, Urbana, Illinois 61801 (United States); Cunningham, Brian T. [Micro and Nanotechnology Laboratory, Department of Electrical and Computer Engineering, University of Illinois at Urbana-Champaign, 208 North Wright Street, Urbana, Illinois 61801 (United States); Department of Bioengineering, University of Illinois at Urbana-Champaign, 1270 Digital Computer Laboratory, MC-278, Urbana, Illinois 61801 (United States)
2015-08-03
Tailored optical output, such as color purity and efficient optical intensity, are critical considerations for displays, particularly in mobile applications. To this end, we demonstrate a replica molded photonic crystal structure with embedded quantum dots. Electrohydrodynamic jet printing is used to control the position of the quantum dots within the device structure. This results in significantly less waste of the quantum dot material than application through drop-casting or spin coating. In addition, the targeted placement of the quantum dots minimizes any emission outside of the resonant enhancement field, which enables an 8× output enhancement and highly polarized emission from the photonic crystal structure.
Synthesis of CdSe Quantum Dots Using Fusarium oxysporum
Takaaki Yamaguchi; Yoshijiro Tsuruda; Tomohiro Furukawa; Lumi Negishi; Yuki Imura; Shohei Sakuda; Etsuro Yoshimura; Michio Suzuki
2016-01-01
CdSe quantum dots are often used in industry as fluorescent materials. In this study, CdSe quantum dots were synthesized using Fusarium oxysporum. The cadmium and selenium concentration, pH, and temperature for the culture of F. oxysporum (Fusarium oxysporum) were optimized for the synthesis, and the CdSe quantum dots obtained from the mycelial cells of F. oxysporum were observed by transmission electron microscopy. Ultra-thin sections of F. oxysporum showed that the CdSe quantum dots were pr...
Core–shell quantum dots: Properties and applications
Energy Technology Data Exchange (ETDEWEB)
Vasudevan, D., E-mail: vasudevand@rediffmail.com [Electrodics and electrocatalysis division, CSIR-CECRI, Karaikudi 630006 (India); Gaddam, Rohit Ranganathan [Amity Institute of Nanotechnology, Amity University, Noida 201301 (India); Trinchi, Adrian; Cole, Ivan [CSIRO Materials Science and Engineering, Clayton South MDC, 3169 (Australia)
2015-07-05
Fluorescent quantum dots (QDs) are semiconducting nanocrystals (NCs) that find numerous applications in areas, such as bio labelling, sensors, lasers, light emitting diodes and medicine. Core–shell quantum dots were developed to improve the photoluminescence efficiency of single quantum dots. Capping their surface with organic ligands as well as their extraction into aqueous media enables their use in sensing applications. The current review highlights the importance and applications of core shell quantum dots as well as their surface modifications and applications in the field of medicine and as sensors for chemical and biochemical analysis.
Single-electron Spin Resonance in a Quadruple Quantum Dot
Otsuka, Tomohiro; Nakajima, Takashi; Delbecq, Matthieu R.; Amaha, Shinichi; Yoneda, Jun; Takeda, Kenta; Allison, Giles; Ito, Takumi; Sugawara, Retsu; Noiri, Akito; Ludwig, Arne; Wieck, Andreas D.; Tarucha, Seigo
2016-08-01
Electron spins in semiconductor quantum dots are good candidates of quantum bits for quantum information processing. Basic operations of the qubit have been realized in recent years: initialization, manipulation of single spins, two qubit entanglement operations, and readout. Now it becomes crucial to demonstrate scalability of this architecture by conducting spin operations on a scaled up system. Here, we demonstrate single-electron spin resonance in a quadruple quantum dot. A few-electron quadruple quantum dot is formed within a magnetic field gradient created by a micro-magnet. We oscillate the wave functions of the electrons in the quantum dots by applying microwave voltages and this induces electron spin resonance. The resonance energies of the four quantum dots are slightly different because of the stray field created by the micro-magnet and therefore frequency-resolved addressable control of each electron spin resonance is possible.
Zhao, Tianshuo; Goodwin, Earl D; Guo, Jiacen; Wang, Han; Diroll, Benjamin T; Murray, Christopher B; Kagan, Cherie R
2016-09-22
Advanced architectures are required to further improve the performance of colloidal PbS heterojunction quantum dot solar cells. Here, we introduce a CdI2-treated CdSe quantum dot buffer layer at the junction between ZnO nanoparticles and PbS quantum dots in the solar cells. We exploit the surface- and size-tunable electronic properties of the CdSe quantum dots to optimize its carrier concentration and energy band alignment in the heterojunction. We combine optical, electrical, and analytical measurements to show that the CdSe quantum dot buffer layer suppresses interface recombination and contributes additional photogenerated carriers, increasing the open-circuit voltage and short-circuit current of PbS quantum dot solar cells, leading to a 25% increase in solar power conversion efficiency.
Borsosfoldi, Z.; Rahman, M.; Larkin, I. A.; Long, A. R.; Davies, J. H.; Weaver, J. M. R.; Holland, M. C.; Williamson, J. G.
1995-06-01
We demonstrate single electron charging in fully controllable nanoscale quantum devices at temperatures above 4 K. Hitherto, single electron devices operating at ``high'' temperatures have been two-terminal, having no control electrode, whereas fully tunable structures such as quantum dots have only shown charging effects at temperatures of 4 K or less. We have fabricated ultrasmall quantum dots on modulation doped heterostructures where the two-dimensional electron gas is less than 30 nm from the surface. Dots with lithographic diameter 150 nm show Coulomb oscillations up to temperatures of 7 K. Higher temperature operation allows potential applications to be considered without the need, for example, of a dilution fridge.
Wang, Yichao; Della Gaspera, Enrico; Carey, Benjamin J.; Atkin, Paul; Berean, Kyle J.; Clark, Rhiannon M.; Cole, Ivan S.; Xu, Zai-Quan; Zhang, Yupeng; Bao, Qiaoliang; Ou, Jian Zhen; Daeneke, Torben; Kalantar-Zadeh, Kourosh
2016-06-01
Developing scalable methods of growing two dimensional molybdenum disulphide (2D MoS2) with strong optical properties, on any desired substrates, is a necessary step towards industrial uptake of this material for optical applications. In this study, Si/SiO2 substrates were functionalised using self-assembled monolayers of three different aminosilanes with various numbers of amine groups and molecular lengths as underlayers for enhancing the adherence of the molybdenum precursor. The tetrahedral [MoS4]2- anion groups from the molybdenum precursor were bonded on these silanised Si/SiO2 substrates afterwards. The substrates were then treated with a combined thermolysis and sulphurisation step. The results showed that silanisation of the substrates using the longest chains and the largest number of amine groups provided a good foundation to grow quasi 2D MoS2 made from adjacent flakes in a mosaic formation. Microscopy and spectroscopy investigations revealed that these quasi 2D MoS2 formed using this long chain aminosilane resulted in flakes with lateral dimensions in micron and submicron ranges composed of adjoining MoS2 pieces of 20 to 60 nm in lateral dimensions, dominantly made of 3 to 5 MoS2 fundamental layers. The obtained quasi 2D MoS2 shows a high internal quantum efficiency of 2.6% associated with the quantum confinement effect and high stoichiometry of the adjoining nanoflakes that form the structure of the sheets. The synthesis technique in this study is reliable and facile and offers a procedure to form large, scalable and patternable quasi 2D MoS2 sheets on various substrates with enhanced optical properties for practical applications.Developing scalable methods of growing two dimensional molybdenum disulphide (2D MoS2) with strong optical properties, on any desired substrates, is a necessary step towards industrial uptake of this material for optical applications. In this study, Si/SiO2 substrates were functionalised using self-assembled monolayers of
Brézin, E
1992-01-01
In the usual matrix-model approach to random discretized two-dimensional manifolds, one introduces n Ising spins on each cell, i.e. a discrete version of 2D quantum gravity coupled to matter with a central charge n/2. The matrix-model consists then of an integral over $2^{n}$ matrices, which we are unable to solve for $n>1$. However for a fixed genus we can expand in the cosmological constant g for arbitrary values of n, and a simple minded analysis of the series yields for n=0,1 and 2 the expected results for the exponent $\\gamma_{string}$ with an amazing precision given the small number of terms that we considered. We then proceed to larger values of n. Simple tests of universality are successfully applied; for instance we obtain the same exponents for n=3 or for one Ising model coupled to a one dimensional target space. The calculations are easily extended to states Potts models, through an integration over $q^{n}$ matrices. We see no sign of the tachyonic instability of the theory, but we have only consid...
Kim, Ju H.; Han, S. Y.; Brooks, J. S.
1999-08-01
We investigate the phenomenon of magnetic breakdown in quasi-two-dimensional organic conductors such as α-(ET)2KHg(SCN)4 and κ-(ET)2Cu(NCS)2 by constructing a tight-binding model based on a realistic band structure which is derived from the crystallographic data. We solve the model numerically to compute the magnetic field dependence of the magnetization and show that the present model accounts naturally for the experimentally observed magnetization oscillation frequencies that are forbidden in the semiclassical picture. The computed values of the fundamental and magnetic breakdown frequencies with no adjustable parameters are close to the experimentally measured values. For completeness, we carry out the computation for both canonical (fixed number of particles) and grand canonical (fixed chemical potential) ensembles, and show that the forbidden frequencies appear in both cases. Hence, the appearance of anomalous frequencies in the de Haas-van Alphen effect has a quantum-mechanical origin and arises from the interplay of electronic states from two partially occupied bands near the Fermi energy as a function of magnetic field. We also compute the temperature dependence of the magnetization and apply ad hoc the Lifshitz-Kosevich analysis to the amplitudes of the Fourier components at moderately high temperatures. This yields effective mass values for α-(ET)2KHg(SCN)4 in good agreement with experimental values.
Effect of phase transition on quantum transport in group-IV two-dimensional U-shape device
Energy Technology Data Exchange (ETDEWEB)
Sadi, Mohammad Abdullah; Gupta, Gaurav, E-mail: a0089293@nus.edu.sg; Liang, Gengchiau [Department of Electrical and Computer Engineering, National University of Singapore, Singapore 117576 (Singapore)
2014-10-21
The effect of phase-transition from the quantum-spin-hall to the band-insulator phase on the transport through a three-terminal U-shape spin-separator has been computationally investigated via non-equilibrium green function formalism. Two-dimensional group-IV elements have been comprehensively appraised as the device material. The device separates the unpolarized current injected at the source-terminal into nearly 100% spin-polarized currents of the opposite polarities at the two drain terminals. The phase-transition activated by the electric-field orthogonal to the device is shown to extensively influence the current magnitude and its spin-polarization, and the effect is stronger for materials with smaller intrinsic spin-orbit coupling. Moreover, the device length and the area under field are shown to critically affect the device characteristics on phase change. It is shown that the same device can be operated as a spin-filter by inducing phase-transition selectively in the channel. The results are important for designing spin-devices from Group-IV monolayers.
Qin, Mingpu; Zhang, Shiwei
2016-01-01
Ground state properties of the Hubbard model on a two-dimensional square lattice are studied by the auxiliary-field quantum Monte Carlo method. Accurate results for energy, double occupancy, effective hopping, magnetization, and momentum distribution are calculated for interaction strengths of U/t from 2 to 8, for a range of densities including half-filling and n = 0.3, 0.5, 0.6, 0.75, and 0.875. At half-filling, the results are numerically exact. Away from half-filling, the constrained path Monte Carlo method is employed to control the sign problem. Our results are obtained with several advances in the computational algorithm, which are described in detail. We discuss the advantages of generalized Hartree-Fock trial wave functions and its connection to pairing wave functions, as well as the interplay with different forms of Hubbard-Stratonovich decompositions. We study the use of different twist angle sets when applying the twist averaged boundary conditions. We propose the use of quasi-random sequences, whi...
Wang, Yichao; Della Gaspera, Enrico; Carey, Benjamin J; Atkin, Paul; Berean, Kyle J; Clark, Rhiannon M; Cole, Ivan S; Xu, Zai-Quan; Zhang, Yupeng; Bao, Qiaoliang; Ou, Jian Zhen; Daeneke, Torben; Kalantar-Zadeh, Kourosh
2016-06-16
Developing scalable methods of growing two dimensional molybdenum disulphide (2D MoS2) with strong optical properties, on any desired substrates, is a necessary step towards industrial uptake of this material for optical applications. In this study, Si/SiO2 substrates were functionalised using self-assembled monolayers of three different aminosilanes with various numbers of amine groups and molecular lengths as underlayers for enhancing the adherence of the molybdenum precursor. The tetrahedral [MoS4](2-) anion groups from the molybdenum precursor were bonded on these silanised Si/SiO2 substrates afterwards. The substrates were then treated with a combined thermolysis and sulphurisation step. The results showed that silanisation of the substrates using the longest chains and the largest number of amine groups provided a good foundation to grow quasi 2D MoS2 made from adjacent flakes in a mosaic formation. Microscopy and spectroscopy investigations revealed that these quasi 2D MoS2 formed using this long chain aminosilane resulted in flakes with lateral dimensions in micron and submicron ranges composed of adjoining MoS2 pieces of 20 to 60 nm in lateral dimensions, dominantly made of 3 to 5 MoS2 fundamental layers. The obtained quasi 2D MoS2 shows a high internal quantum efficiency of 2.6% associated with the quantum confinement effect and high stoichiometry of the adjoining nanoflakes that form the structure of the sheets. The synthesis technique in this study is reliable and facile and offers a procedure to form large, scalable and patternable quasi 2D MoS2 sheets on various substrates with enhanced optical properties for practical applications.
Quantum-Dot-Based Telecommunication-Wavelength Quantum Relay
Huwer, J.; Stevenson, R. M.; Skiba-Szymanska, J.; Ward, M. B.; Shields, A. J.; Felle, M.; Farrer, I.; Ritchie, D. A.; Penty, R. V.
2017-08-01
The development of quantum relays for long-haul and attack-proof quantum communication networks operating with weak coherent laser pulses requires entangled photon sources at telecommunication wavelengths with intrinsic single-photon emission for most practical implementations. Using a semiconductor quantum dot emitting entangled photon pairs in the telecommunication O band, we demonstrate a quantum relay fulfilling both of these conditions. The system achieves a maximum fidelity of 94.5% for implementation of a standard four-state protocol with input states generated by a laser. We further investigate robustness against frequency detuning of the narrow-band input and perform process tomography of the teleporter, revealing operation for arbitrary pure input states, with an average gate fidelity of 83.6%. The results highlight the potential of semiconductor light sources for compact and robust quantum-relay technology that is compatible with existing communication infrastructures.
Wu, Wei; Xu, Jing-Bo
2016-08-01
We investigate the quantum phase transitions of spin systems in one and two dimensions by employing trace distance and multipartite entanglement along with the real-space quantum renormalization group method. As illustration examples, a one-dimensional and a two-dimensional XY models are considered. It is shown that the quantum phase transitions of these spin-chain systems can be revealed by the singular behaviors of the first derivatives of renormalized trace distance and multipartite entanglement in the thermodynamics limit. Moreover, we find that the renormalized trace distance and multipartite entanglement obey certain universal exponential-type scaling laws in the vicinity of the quantum critical points.
Boda, Aalu; Kumar, D. Sanjeev; Sankar, I. V.; Chatterjee, Ashok
2016-11-01
The problem of a parabolically confined two-dimensional semiconductor GaAs quantum dot with two interacting electrons in the presence of an external magnetic field and the spin-Zeeman interaction is studied using a method of numerical diagonalization. The energy spectrum is calculated as a function of the magnetic field. The magnetic moment (M) and the magnetic susceptibility (χ) show zero temperature diamagnetic peaks due to the exchange induced singlet-triplet transitions. The position and the number of these peaks depend both on the confinement strength of the quantum dot and the strength of the electron-electron interaction (β) .
Quantum dots for next-generation photovoltaics
Directory of Open Access Journals (Sweden)
Octavi E. Semonin
2012-11-01
Full Text Available Colloidal quantum-confined semiconductor nanostructures are an emerging class of functional material that are being developed for novel solar energy conversion strategies. One of the largest losses in a bulk or thin film solar cell occurs within a few picoseconds after the photon is absorbed, as photons with energy larger than the semiconductor bandgap produce charge-carriers with excess kinetic energy, which is then dissipated via phonon emission. Semiconductor nanostructures, where at least one dimension is small enough to produce quantum confinement effects, provide new pathways for controlling energy flow and therefore have the potential to increase the efficiency of the primary photoconversion step. In this review, we provide the current status of research efforts towards utilizing the unique properties of colloidal quantum dots (nanocrystals confined in three dimensions in prototype solar cells and demonstrate that these unique systems have the potential to bypass the Shockley-Queisser single-junction limit for solar photon conversion.
Hybrid passivated colloidal quantum dot solids
Ip, Alexander H.; Thon, Susanna M.; Hoogland, Sjoerd; Voznyy, Oleksandr; Zhitomirsky, David; Debnath, Ratan; Levina, Larissa; Rollny, Lisa R.; Carey, Graham H.; Fischer, Armin; Kemp, Kyle W.; Kramer, Illan J.; Ning, Zhijun; Labelle, André J.; Chou, Kang Wei; Amassian, Aram; Sargent, Edward H.
2012-09-01
Colloidal quantum dot (CQD) films allow large-area solution processing and bandgap tuning through the quantum size effect. However, the high ratio of surface area to volume makes CQD films prone to high trap state densities if surfaces are imperfectly passivated, promoting recombination of charge carriers that is detrimental to device performance. Recent advances have replaced the long insulating ligands that enable colloidal stability following synthesis with shorter organic linkers or halide anions, leading to improved passivation and higher packing densities. Although this substitution has been performed using solid-state ligand exchange, a solution-based approach is preferable because it enables increased control over the balance of charges on the surface of the quantum dot, which is essential for eliminating midgap trap states. Furthermore, the solution-based approach leverages recent progress in metal:chalcogen chemistry in the liquid phase. Here, we quantify the density of midgap trap states in CQD solids and show that the performance of CQD-based photovoltaics is now limited by electron-hole recombination due to these states. Next, using density functional theory and optoelectronic device modelling, we show that to improve this performance it is essential to bind a suitable ligand to each potential trap site on the surface of the quantum dot. We then develop a robust hybrid passivation scheme that involves introducing halide anions during the end stages of the synthesis process, which can passivate trap sites that are inaccessible to much larger organic ligands. An organic crosslinking strategy is then used to form the film. Finally, we use our hybrid passivated CQD solid to fabricate a solar cell with a certified efficiency of 7.0%, which is a record for a CQD photovoltaic device.
Hybrid passivated colloidal quantum dot solids
Ip, Alex
2012-07-29
Colloidal quantum dot (CQD) films allow large-area solution processing and bandgap tuning through the quantum size effect. However, the high ratio of surface area to volume makes CQD films prone to high trap state densities if surfaces are imperfectly passivated, promoting recombination of charge carriers that is detrimental to device performance. Recent advances have replaced the long insulating ligands that enable colloidal stability following synthesis with shorter organic linkers or halide anions, leading to improved passivation and higher packing densities. Although this substitution has been performed using solid-state ligand exchange, a solution-based approach is preferable because it enables increased control over the balance of charges on the surface of the quantum dot, which is essential for eliminating midgap trap states. Furthermore, the solution-based approach leverages recent progress in metal:chalcogen chemistry in the liquid phase. Here, we quantify the density of midgap trap states in CQD solids and show that the performance of CQD-based photovoltaics is now limited by electrong-"hole recombination due to these states. Next, using density functional theory and optoelectronic device modelling, we show that to improve this performance it is essential to bind a suitable ligand to each potential trap site on the surface of the quantum dot. We then develop a robust hybrid passivation scheme that involves introducing halide anions during the end stages of the synthesis process, which can passivate trap sites that are inaccessible to much larger organic ligands. An organic crosslinking strategy is then used to form the film. Finally, we use our hybrid passivated CQD solid to fabricate a solar cell with a certified efficiency of 7.0%, which is a record for a CQD photovoltaic device. © 2012 Macmillan Publishers Limited. All rights reserved.
Nonrenewal statistics in transport through quantum dots
Ptaszyński, Krzysztof
2017-01-01
The distribution of waiting times between successive tunneling events is an already established method to characterize current fluctuations in mesoscopic systems. Here, I investigate mechanisms generating correlations between subsequent waiting times in two model systems, a pair of capacitively coupled quantum dots and a single-level dot attached to spin-polarized leads. Waiting time correlations are shown to give insight into the internal dynamics of the system; for example they allow distinction between different mechanisms of the noise enhancement. Moreover, the presence of correlations breaks the validity of the renewal theory. This increases the number of independent cumulants of current fluctuation statistics, thus providing additional sources of information about the transport mechanism. I also propose a method for inferring the presence of waiting time correlations based on low-order current correlation functions. This method gives a way to extend the analysis of nonrenewal current fluctuations to the systems for which single-electron counting is not experimentally feasible. The experimental relevance of the findings is also discussed; for example reanalysis of previous results concerning transport in quantum dots is suggested.
Production and targeting of monovalent quantum dots.
Seo, Daeha; Farlow, Justin; Southard, Kade; Jun, Young-Wook; Gartner, Zev J
2014-10-23
The multivalent nature of commercial quantum dots (QDs) and the difficulties associated with producing monovalent dots have limited their applications in biology, where clustering and the spatial organization of biomolecules is often the object of study. We describe here a protocol to produce monovalent quantum dots (mQDs) that can be accomplished in most biological research laboratories via a simple mixing of CdSe/ZnS core/shell QDs with phosphorothioate DNA (ptDNA) of defined length. After a single ptDNA strand has wrapped the QD, additional strands are excluded from the surface. Production of mQDs in this manner can be accomplished at small and large scale, with commercial reagents, and in minimal steps. These mQDs can be specifically directed to biological targets by hybridization to a complementary single stranded targeting DNA. We demonstrate the use of these mQDs as imaging probes by labeling SNAP-tagged Notch receptors on live mammalian cells, targeted by mQDs bearing a benzylguanine moiety.
Amphoteric CdSe nanocrystalline quantum dots.
Islam, Mohammad A
2008-06-25
The nanocrystal quantum dot (NQD) charge states strongly influence their electrical transport properties in photovoltaic and electroluminescent devices, optical gains in NQD lasers, and the stability of the dots in thin films. We report a unique electrostatic nature of CdSe NQDs, studied by electrophoretic methods. When we submerged a pair of metal electrodes, in a parallel plate capacitor configuration, into a dilute solution of CdSe NQDs in hexane, and applied a DC voltage across the pair, thin films of CdSe NQDs were deposited on both the positive and the negative electrodes. Extensive characterizations including scanning electron microscopy (SEM), atomic force microscopy (AFM), Fourier transform infrared (FTIR) and Raman studies revealed that the films on both the positive and the negative electrodes were identical in every respect, clearly indicating that: (1) a fraction (<1%) of the CdSe NQDs in free form in hexane solution are charged and, more importantly, (2) there are equal numbers of positive and negative CdSe NQDs in the hexane solution. Experiments also show that the number of deposited dots is at least an order of magnitude higher than the number of initially charged dots, indicating regeneration. We used simple thermodynamics to explain such amphoteric nature and the charging/regeneration of the CdSe NQDs.
A two-dimensional Dirac fermion microscope
Bøggild, Peter; Caridad, José M.; Stampfer, Christoph; Calogero, Gaetano; Papior, Nick Rübner; Brandbyge, Mads
2017-06-01
The electron microscope has been a powerful, highly versatile workhorse in the fields of material and surface science, micro and nanotechnology, biology and geology, for nearly 80 years. The advent of two-dimensional materials opens new possibilities for realizing an analogy to electron microscopy in the solid state. Here we provide a perspective view on how a two-dimensional (2D) Dirac fermion-based microscope can be realistically implemented and operated, using graphene as a vacuum chamber for ballistic electrons. We use semiclassical simulations to propose concrete architectures and design rules of 2D electron guns, deflectors, tunable lenses and various detectors. The simulations show how simple objects can be imaged with well-controlled and collimated in-plane beams consisting of relativistic charge carriers. Finally, we discuss the potential of such microscopes for investigating edges, terminations and defects, as well as interfaces, including external nanoscale structures such as adsorbed molecules, nanoparticles or quantum dots.
A two-dimensional Dirac fermion microscope.
Bøggild, Peter; Caridad, José M; Stampfer, Christoph; Calogero, Gaetano; Papior, Nick Rübner; Brandbyge, Mads
2017-06-09
The electron microscope has been a powerful, highly versatile workhorse in the fields of material and surface science, micro and nanotechnology, biology and geology, for nearly 80 years. The advent of two-dimensional materials opens new possibilities for realizing an analogy to electron microscopy in the solid state. Here we provide a perspective view on how a two-dimensional (2D) Dirac fermion-based microscope can be realistically implemented and operated, using graphene as a vacuum chamber for ballistic electrons. We use semiclassical simulations to propose concrete architectures and design rules of 2D electron guns, deflectors, tunable lenses and various detectors. The simulations show how simple objects can be imaged with well-controlled and collimated in-plane beams consisting of relativistic charge carriers. Finally, we discuss the potential of such microscopes for investigating edges, terminations and defects, as well as interfaces, including external nanoscale structures such as adsorbed molecules, nanoparticles or quantum dots.
Quantum Dots: An Experiment for Physical or Materials Chemistry
Winkler, L. D.; Arceo, J. F.; Hughes, W. C.; DeGraff, B. A.; Augustine, B. H.
2005-01-01
An experiment is conducted for obtaining quantum dots for physical or materials chemistry. This experiment serves to both reinforce the basic concept of quantum confinement and providing a useful bridge between the molecular and solid-state world.
Resonance fluorescence from a telecom-wavelength quantum dot
Al-Khuzheyri, R; Huwer, J; Santana, T S; Szymanska, J Skiba-; Felle, M; Ward, M B; Stevenson, R M; Farrer, I; Tanner, M G; Hadfield, R H; Ritchie, D A; Shields, A J; Gerardot, B D
2016-01-01
We report on resonance fluorescence from a single quantum dot emitting at telecom wavelengths. We perform high-resolution spectroscopy and observe the Mollow triplet in the Rabi regime--a hallmark of resonance fluorescence. The measured resonance-fluorescence spectra allow us to rule out pure dephasing as a significant decoherence mechanism in these quantum dots. Combined with numerical simulations, the experimental results provide robust characterisation of charge noise in the environment of the quantum dot. Resonant control of the quantum dot opens up new possibilities for on-demand generation of indistinguishable single photons at telecom wavelengths as well as quantum optics experiments and direct manipulation of solid-state qubits in telecom-wavelength quantum dots.
Coherent Dynamics of Quantum Dots in Photonic-Crystal Cavities
DEFF Research Database (Denmark)
Madsen, Kristian Høeg
deviations. Similar measurements on a quantum dot in a photonic-crystal cavity sow a Rabi splitting on resonance, while time-resolved measurements prove that the system is in the weak coupling regime. Whle tuning the quantum dot through resonance of the high-Q mode we observe a strong and surprisingly...... Successfully model the decay rates with a microscopic model that allows us to for the first time extract the effective phonon density of states, which we can model with bulk phonons. Studies on a quantum dot detuned from a low-Q mode of a photonic-crystal cavity show a high collection efficiency at the first......In this thesis we have performed quantum-electrodynamics experiments on quantum dots embedded in photonic-crystal cavities. We perform a quantitative comparison of the decay dynamics and emission spectra of quantum dots embedded in a micropillar cavity and a photonic-crystal cavity. The light...
Electrostatically defined silicon quantum dots with counted antimony donor implants
Energy Technology Data Exchange (ETDEWEB)
Singh, M., E-mail: msingh@sandia.gov; Luhman, D. R.; Lilly, M. P. [Sandia National Laboratories, Albuquerque, New Mexico 87185 (United States); Center for Integrated Nanotechnologies, Sandia National Laboratories, Albuquerque, New Mexico 87175 (United States); Pacheco, J. L.; Perry, D.; Garratt, E.; Ten Eyck, G.; Bishop, N. C.; Wendt, J. R.; Manginell, R. P.; Dominguez, J.; Pluym, T.; Bielejec, E.; Carroll, M. S. [Sandia National Laboratories, Albuquerque, New Mexico 87185 (United States)
2016-02-08
Deterministic control over the location and number of donors is crucial to donor spin quantum bits (qubits) in semiconductor based quantum computing. In this work, a focused ion beam is used to implant antimony donors in 100 nm × 150 nm windows straddling quantum dots. Ion detectors are integrated next to the quantum dots to sense the implants. The numbers of donors implanted can be counted to a precision of a single ion. In low-temperature transport measurements, regular Coulomb blockade is observed from the quantum dots. Charge offsets indicative of donor ionization are also observed in devices with counted donor implants.
Photon Cascade from a Single Crystal Phase Nanowire Quantum Dot
DEFF Research Database (Denmark)
Bouwes Bavinck, Maaike; Jöns, Klaus D; Zieliński, Michal
2016-01-01
unprecedented potential to be controlled with atomic layer accuracy without random alloying. We show for the first time that crystal phase quantum dots are a source of pure single-photons and cascaded photon-pairs from type II transitions with excellent optical properties in terms of intensity and line width...... quantum optical properties for single photon application and quantum optics.......We report the first comprehensive experimental and theoretical study of the optical properties of single crystal phase quantum dots in InP nanowires. Crystal phase quantum dots are defined by a transition in the crystallographic lattice between zinc blende and wurtzite segments and therefore offer...
2014-01-01
We investigate coherent single surface-plasmon transport in a metal nanowire strongly coupled to two colloidal quantum dots. Analytical expressions are obtained for the transmission and reflection coefficients by solving the corresponding eigenvalue equation. Remote entanglement of the wave functions of the two quantum dots can be created if the inter-dot distance is equal to a multiple half-wavelength of the surface plasmon. Furthermore, by applying classical laser pulses to the quantum dots...
Quantum state preparation in semiconductor dots by adiabatic rapid passage
Wu, Yanwen; Piper, I.M.; Ediger, M.; Brereton, P.; Schmidgall, E. R.; Hugues, M.; Hopkinson, M.; Phillips, R.T.
2010-01-01
Preparation of a specific quantum state is a required step for a variety of proposed practical uses of quantum dynamics. We report an experimental demonstration of optical quantum state preparation in a semiconductor quantum dot with electrical readout, which contrasts with earlier work based on Rabi flopping in that the method is robust with respect to variation in the optical coupling. We use adiabatic rapid passage, which is capable of inverting single dots to a specified upper level. We d...
Coupled quantum dot-ring structures by droplet epitaxy
Energy Technology Data Exchange (ETDEWEB)
Somaschini, C; Bietti, S; Koguchi, N; Sanguinetti, S, E-mail: stefano.sanguinetti@unimib.it [L-NESS and Dipartimento di Scienza dei Materiali, Universita di Milano Bicocca, Via Cozzi 53, I-20125 Milano (Italy)
2011-05-06
The fabrication, by pure self-assembly, of GaAs/AlGaAs dot-ring quantum nanostructures is presented. The growth is performed via droplet epitaxy, which allows for the fine control, through As flux and substrate temperature, of the crystallization kinetics of nanometer scale metallic Ga reservoirs deposited on the surface. Such a procedure permits the combination of quantum dots and quantum rings into a single, multi-functional, complex quantum nanostructure.
Colloidal Quantum Dot Photovoltaics: A Path Forward
Kramer, Illan J.
2011-11-22
Colloidal quantum dots (CQDs) offer a path toward high-efficiency photovoltaics based on low-cost materials and processes. Spectral tunability via the quantum size effect facilitates absorption of specific wavelengths from across the sun\\'s broad spectrum. CQD materials\\' ease of processing derives from their synthesis, storage, and processing in solution. Rapid advances have brought colloidal quantum dot photovoltaic solar power conversion efficiencies of 6% in the latest reports. These achievements represent important first steps toward commercially compelling performance. Here we review advances in device architecture and materials science. We diagnose the principal phenomenon-electronic states within the CQD film band gap that limit both current and voltage in devices-that must be cured for CQD PV devices to fulfill their promise. We close with a prescription, expressed as bounds on the density and energy of electronic states within the CQD film band gap, that should allow device efficiencies to rise to those required for the future of the solar energy field. © 2011 American Chemical Society.
Nano-laser on silicon quantum dots
Huang, Wei-Qi; Liu, Shi-Rong; Qin, Chao-Jian; Lü, Quan; Xu, Li
2011-04-01
A new conception of nano-laser is proposed in which depending on the size of nano-clusters (silicon quantum dots (QD)), the pumping level of laser can be tuned by the quantum confinement (QC) effect, and the population inversion can be formed between the valence band and the localized states in gap produced from the surface bonds of nano-clusters. Here we report the experimental demonstration of nano-laser on silicon quantum dots fabricated by nanosecond pulse laser. The peaks of stimulated emission are observed at 605 nm and 693 nm. Through the micro-cavity of nano-laser, a full width at half maximum of the peak at 693 nm can reach to 0.5 nm. The theoretical model and the experimental results indicate that it is a necessary condition for setting up nano-laser that the smaller size of QD (d nano-laser will be limited in the range of 1.7-2.3 eV generally due to the position of the localized states in gap, which is in good agreement between the experiments and the theory.
Nonequilibrium Electron Transport Through a Quantum Dot from Kubo Formula
Institute of Scientific and Technical Information of China (English)
L(U) Rong; ZHANG Guang-Ming
2005-01-01
Based on the Kubo formula for an electron tunneling junction, we revisit the nonequilibrium transport properties through a quantum dot. Since the Fermi level of the quantum dot is set by the conduction electrons of the leads, we calculate the electron current from the left side by assuming the quantum dot coupled to the right lead as another side of the tunneling junction, and the other way round is used to calculate the current from the right side. By symmetrizing these two currents, an effective local density states on the dot can be obtained, and is discussed at high and low temperatures, respectively.
Implementing of Quantum Cloning with Spatially Separated Quantum Dot Spins
Wen, Jing-Ji; Yeon, Kyu-Hwang; Du, Xin; Lv, Jia; Wang, Ming; Wang, Hong-Fu; Zhang, Shou
2016-07-01
We propose some schemes for implementing optimal symmetric (asymmetric) 1 → 2 universal quantum cloning, optimal symmetric (asymmetric) 1 → 2 phase-covariant cloning, optimal symmetric 1 → 3 economical phase-covariant cloning and optimal symmetric 1 → 3 economical real state cloning with spatially separated quantum dot spins by choosing the single-qubit rotation angles appropriately. The decoherences of the spontaneous emission of QDs, cavity decay and fiber loss are suppressed since the effective long-distance off-resonant interaction between two distant QDs is mediated by the vacuum fields of the fiber and cavity, and during the whole process no system is excited.
Systematic optimization of quantum junction colloidal quantum dot solar cells
Liu, Huan
2012-01-01
The recently reported quantum junction architecture represents a promising approach to building a rectifying photovoltaic device that employs colloidal quantum dot layers on each side of the p-n junction. Here, we report an optimized quantum junction solar cell that leverages an improved aluminum zinc oxide electrode for a stable contact to the n-side of the quantum junction and silver doping of the p-layer that greatly enhances the photocurrent by expanding the depletion region in the n-side of the device. These improvements result in greater stability and a power conversion efficiency of 6.1 under AM1.5 simulated solar illumination. © 2012 American Institute of Physics.
Quantum model for mode locking in pulsed semiconductor quantum dots
Beugeling, W.; Uhrig, Götz S.; Anders, Frithjof B.
2016-12-01
Quantum dots in GaAs/InGaAs structures have been proposed as a candidate system for realizing quantum computing. The short coherence time of the electronic quantum state that arises from coupling to the nuclei of the substrate is dramatically increased if the system is subjected to a magnetic field and to repeated optical pulsing. This enhancement is due to mode locking: oscillation frequencies resonant with the pulsing frequencies are enhanced, while off-resonant oscillations eventually die out. Because the resonant frequencies are determined by the pulsing frequency only, the system becomes immune to frequency shifts caused by the nuclear coupling and by slight variations between individual quantum dots. The effects remain even after the optical pulsing is terminated. In this work, we explore the phenomenon of mode locking from a quantum mechanical perspective. We treat the dynamics using the central-spin model, which includes coupling to 10-20 nuclei and incoherent decay of the excited electronic state, in a perturbative framework. Using scaling arguments, we extrapolate our results to realistic system parameters. We estimate that the synchronization to the pulsing frequency needs time scales in the order of 1 s .
Mesoscopic quantum interference experiments in InGaAs and GaAs two-dimensional systems
Ren, Shaola
The study of quantum interference in solid-state systems yields insight in fundamental properties of mesoscopic systems. Electron quantum interference constitutes an important method to explore mesoscopic physics and quantum decoherence. This dissertation focuses on two-dimensional (2D) electron systems in delta-Si doped n-type In0:64Ga0:36As/In 0:45Al0:55As, 2D hole systems in Si-doped p-type GaAs/Al 0:35Ga0:65As and C-doped p-type GaAs/Al0:24Ga 0:76As heterostructures. The low temperature experiments study the magnetotransport of nano- and micro-scale lithographically defined devices fabricated on the heterostructures. These devices include a single ring interferometer and a ring interferometer array in 2D electron system, Hall bar geometries and narrow wires in 2D hole systems. The single ring interferometer yields pronounced Aharonov-Bohm (AB) oscillations with magnetic flux periodicity of h/e over a wide range of magnetic field. The periodicity was confirmed by Fourier transformation of the oscillations. The AB oscillation amplitude shows a quasi-periodic modulation over applied magnetic field due to local magnetic flux threading through the interferometer arms. Further study of current and temperature dependence of the amplitude of the oscillations indicates that the Thouless energy forms the measure of excitation energies giving quantum decoherence. An in-plane magnetic field was applied to the single ring interferometer to study the Berry's phase and the Aharonov-Casher effect. The ring interferometer array yields both AB oscillations and Altshuler-Aronov-Spivak (AAS) oscillations, the latter with magnetic flux periodicity of h/2e. The AAS oscillations require time-reversal symmetry and hence can be used to qualify time-reversal symmetry breaking. More importantly, the fundamental mesoscopic dephasing length associated with time-reversal symmetry breaking under applied magnetic field, an effective magnetic length, can be obtained by the analysis of the AAS
A Nanowire-Based Plasmonic Quantum Dot Laser.
Ho, Jinfa; Tatebayashi, Jun; Sergent, Sylvain; Fong, Chee Fai; Ota, Yasutomo; Iwamoto, Satoshi; Arakawa, Yasuhiko
2016-04-13
Quantum dots enable strong carrier confinement and exhibit a delta-function like density of states, offering significant improvements to laser performance and high-temperature stability when used as a gain medium. However, quantum dot lasers have been limited to photonic cavities that are diffraction-limited and further miniaturization to meet the demands of nanophotonic-electronic integration applications is challenging based on existing designs. Here we introduce the first quantum dot-based plasmonic laser to reduce the cross-sectional area of nanowire quantum dot lasers below the cutoff limit of photonic modes while maintaining the length in the order of the lasing wavelength. Metal organic chemical vapor deposition grown GaAs-AlGaAs core-shell nanowires containing InGaAs quantum dot stacks are placed directly on a silver film, and lasing was observed from single nanowires originating from the InGaAs quantum dot emission into the low-loss higher order plasmonic mode. Lasing threshold pump fluences as low as ∼120 μJ/cm(2) was observed at 7 K, and lasing was observed up to 125 K. Temperature stability from the quantum dot gain, leading to a high characteristic temperature was demonstrated. These results indicate that high-performance, miniaturized quantum dot lasers can be realized with plasmonics.
High-resolution photoluminescence studies of single semiconductor quantum dots
DEFF Research Database (Denmark)
Leosson, Kristjan; Østergaard, John Erland; Jensen, Jacob Riis
2000-01-01
Semiconductor quantum dots, especially those formed by self-organized growth, are considered a promising material system for future optical devices [1] and the optical properties of quantum dot ensembles have been investigated in detail over the past years. Recently, considerable interest has dev...
Exciton dephasing in single InGaAs quantum dots
DEFF Research Database (Denmark)
Leosson, Kristjan; Østergaard, John Erland; Jensen, Jacob Riis;
2000-01-01
. The homogeneous and inhomogeneous broadening of InGaAs quantum dot luminescence is of central importance for the potential application of this material system in optoelectronic devices. Recent measurements of MOCVD-grown InAs/InGaAs quantum dots indicate a large homogeneous broadening at room temperature due...
Negative Trions Trapped by a Spherical Parabolic Quantum Dot
Institute of Scientific and Technical Information of China (English)
无
2006-01-01
In this paper, a negatively charged exciton trapped by a spherical parabolic quantum dot has been investigated. The energy spectra of low-lying states are calculated by means of matrix diagonalization. The important feature of the low-lying states of the negatively charged excitons in a spherical quantum dot is obtained via an analysis of the energy spectra.
Imaging vasculature and lymphatic flow in mice using quantum dots
DEFF Research Database (Denmark)
Ballou, Byron; Ernst, Lauren A.; Andreko, Susan
2009-01-01
Quantum dots are ideal probes for fluorescent imaging of vascular and lymphatic tissues. On injection into appropriate sites, red- and near-infrared-emitting quantum dots provide excellent definition of vasculature, lymphoid organs, and lymph nodes draining both normal tissues and tumors. We detail...
Imaging vasculature and lymphatic flow in mice using quantum dots
DEFF Research Database (Denmark)
Ballou, Byron; Ernst, Lauren A.; Andreko, Susan
2009-01-01
Quantum dots are ideal probes for fluorescent imaging of vascular and lymphatic tissues. On injection into appropriate sites, red- and near-infrared-emitting quantum dots provide excellent definition of vasculature, lymphoid organs, and lymph nodes draining both normal tissues and tumors. We deta...
Fast synthesize ZnO quantum dots via ultrasonic method.
Yang, Weimin; Zhang, Bing; Ding, Nan; Ding, Wenhao; Wang, Lixi; Yu, Mingxun; Zhang, Qitu
2016-05-01
Green emission ZnO quantum dots were synthesized by an ultrasonic sol-gel method. The ZnO quantum dots were synthesized in various ultrasonic temperature and time. Photoluminescence properties of these ZnO quantum dots were measured. Time-resolved photoluminescence decay spectra were also taken to discover the change of defects amount during the reaction. Both ultrasonic temperature and time could affect the type and amount of defects in ZnO quantum dots. Total defects of ZnO quantum dots decreased with the increasing of ultrasonic temperature and time. The dangling bonds defects disappeared faster than the optical defects. Types of optical defects first changed from oxygen interstitial defects to oxygen vacancy and zinc interstitial defects. Then transformed back to oxygen interstitial defects again. The sizes of ZnO quantum dots would be controlled by both ultrasonic temperature and time as well. That is, with the increasing of ultrasonic temperature and time, the sizes of ZnO quantum dots first decreased then increased. Moreover, concentrated raw materials solution brought larger sizes and more optical defects of ZnO quantum dots.
Electron transport and coherence in semiconductor quantum dots and rings
Van der Wiel, W.G.
2002-01-01
A number of experiments on electron transport and coherence in semiconductor vertical and lateral quantum dots and semiconductor rings is described. Quantum dots are often referred to as "artificial atoms", because of their similarities with real atoms. Examples of such atom-like properties that
Synthesis, Photoluminescence and Bio-Targeting Applications of Blue Graphene Quantum Dots.
Wang, Jigang; Zhou, Ji; Zhou, Wenhua; Shi, Jilong; Ma, Lun; Chen, Wei; Wang, Yongsheng; He, Dawei; Fu, Ming; Zhang, Yongna
2016-04-01
Chemical derived graphene oxide, an atomically thin sheet of graphite with two-dimensional construction, offers interesting physical, electronic, thermal, chemical, and mechanical properties that are currently being explored for advanced physics electronics, membranes, and composites. Herein, we study graphene quantum dots (GQD) with the blue photoluminescence under various parameters. The GQD samples were prepared at different temperatures, and the blue photoluminescence intensity of the solution improved radically as the heating temperatures increased. Concerning PL peak and intensity of the quantum dots, the results demonstrated dependence on time under heating, temperature of heating, and pH adjusted by the addition of sodium hydroxide. After hydrothermal synthesis routes, the functional groups of graphene oxide were altered the morphology showed the stacking configuration, and self-assembled structure of the graphene sheets with obvious wrinkles appeared at the edge structures. In addition, absorption, PL, and PLE spectra of the graphene quantum dots increase with different quantities of sodium hydroxide added. Finally, using GQD to target PNTIA cells was carried out successfully. High uptake efficiency and no cytotoxic effects indicate graphene quantum dots can be suitable for bio-targeting.
Coupling self-assembled quantum dots to nanostructures
Badolato, Antonio
Self-assembled quantum dot (QD) grown by molecular beam epitaxy implements the ultimate quantum confined structure in the solid-state. Because electrons are confined in all three dimensions, QDs have shown delta-function-like energy dependence of the density of states. The identification of QDs as artificial atoms has been proven by the observation of fundamental exciton emission with perfect photon antibunching and with a linewidth limited by spontaneous emission. As artificial atoms that can be monolithically integrated with other functional devices in the setting of semiconductor technology, QDs have been the source of inspiration of several novel quantum devices. Nonetheless, QD self-assemble on random nucleation sites, whereas many proposals require precise positioning of a single QD. In this thesis, two new elements of design and control for coupling single QDs to single nanostructure will be presented: (i) a technique to control ab-initio the site nucleation of a single QD and (ii) a deterministic approach to the coupling of single QDs to single nanocavity modes. Chapter 1 is dedicated to a theoretical overview of the QD system, first, as a solid-state heterostructure that confines electrons and, second, as an artificial atom interacting with confined photons. Chapter 2 presents a technique to grow highly ordered QD arrays by engineering subsurface periodic strain templates. This technique achieved almost perfect registering of single QDs into a two-dimensional lattice. In Chapter 3 a deterministic approach to the realization of solid-state cavity quantum electrodynamics (QED) systems is demonstrated. Based on a precise spatial and spectral matching between a single QD and a PC microcavity, this approach yielded cavity QED effects (such as Purcell effect) in all fabricated nanostructures.
de Forges de Parny, L.; Rousseau, V. G.
2017-01-01
We study the ground state and the thermal phase diagram of a two-species Bose-Hubbard model, with U(1 ) ×Z2 symmetry, describing atoms and molecules on a two-dimensional optical lattice interacting via a Feshbach resonance. Using quantum Monte Carlo simulations and mean-field theory, we show that the conversion between the two species, coherently coupling the atomic and molecular states, has a crucial impact on the Mott-superfluid transition and stabilizes an insulating phase with a gap controlled by the conversion term—the Feshbach insulator—instead of a standard Mott-insulating phase. Depending on the detuning between atoms and molecules, this model exhibits three phases: the Feshbach insulator, a molecular condensate coexisting with noncondensed atoms, and a mixed atomic-molecular condensate. Employing finite-size scaling analysis, we observe three-dimensional (3D) X Y (3D Ising) transition when U(1 ) (Z2) symmetry is broken, whereas the transition is first order when both U(1 ) and Z2 symmetries are spontaneously broken. The finite-temperature phase diagram is also discussed. The thermal disappearance of the molecular superfluid leads to a Berezinskii-Kosterlitz-Thouless transition with unusual universal jump in the superfluid density. The loss of the quasi-long-range coherence of the mixed atomic and molecular superfluid is more subtle since only atoms exhibit conventional Berezinskii-Kosterlitz-Thouless criticality. We also observe a signal compatible with a classical first-order transition between the mixed superfluid and the normal Bose liquid at low temperature.
Quantum computation with nuclear spins in quantum dots
Energy Technology Data Exchange (ETDEWEB)
Christ, H.
2008-01-24
The role of nuclear spins for quantum information processing in quantum dots is theoretically investigated in this thesis. Building on the established fact that the most strongly coupled environment for the potential electron spin quantum bit are the surrounding lattice nuclear spins interacting via the hyperfine interaction, we turn this vice into a virtue by designing schemes for harnessing this strong coupling. In this perspective, the ensemble of nuclear spins can be considered an asset, suitable for an active role in quantum information processing due to its intrinsic long coherence times. We present experimentally feasible protocols for the polarization, i.e. initialization, of the nuclear spins and a quantitative solution to our derived master equation. The polarization limiting destructive interference effects, caused by the collective nature of the nuclear coupling to the electron spin, are studied in detail. Efficient ways of mitigating these constraints are presented, demonstrating that highly polarized nuclear ensembles in quantum dots are feasible. At high, but not perfect, polarization of the nuclei the evolution of an electron spin in contact with the spin bath can be efficiently studied by means of a truncation of the Hilbert space. It is shown that the electron spin can function as a mediator of universal quantum gates for collective nuclear spin qubits, yielding a promising architecture for quantum information processing. Furthermore, we show that at high polarization the hyperfine interaction of electron and nuclear spins resembles the celebrated Jaynes-Cummings model of quantum optics. This result opens the door for transfer of knowledge from the mature field of quantum computation with atoms and photons. Additionally, tailored specifically for the quantum dot environment, we propose a novel scheme for the generation of highly squeezed collective nuclear states. Finally we demonstrate that even an unprepared completely mixed nuclear spin
Gates controlled parallel-coupled bilayer graphene double quantum dot
Wang, Lin-Jun; Wei, Da; Cao, Gang; Tu, Tao; Xiao, Ming; Guo, Guang-Can; Chang, A M
2011-01-01
Here we report the fabrication and quantum transport measurements of gates controlled parallel-coupled bilayer graphene double quantum dot. It is shown that the interdot coupling strength of the parallel double dots can be effectively tuned from weak to strong regime by both the in-plane plunger gates and back gate. All the relevant energy scales and parameters of the bilayer graphene parallel-coupled double dot can be extracted from the honeycomb charge stability diagrams revealed through the transport measurements.
Self-polarization in spherical quantum dot
Directory of Open Access Journals (Sweden)
Stojanović Dušanka P.
2015-01-01
Full Text Available The electronic structures of CdS quantum dot (QD with dielectric mismatch are calculated. Poisson equation is solved analitically in case of point charge placed inside semiconductor sphere embeded in dielectric matrix in case of different values of the dielectric permittivity of QD and matrix. The validity of the effective mass approximation for the conduction band is assumed. Schrödinger equation for one electron is solved analitically. On the basis of the Poisson equation solution self potential is examined and used as perturbation to calculate the self-polarization effect.
Graphene Quantum Dots for Theranostics and Bioimaging.
Schroeder, Kathryn L; Goreham, Renee V; Nann, Thomas
2016-10-01
Since their advent in the early 1990s, nanomaterials hold promise to constitute improved technologies in the biomedical area. In particular, graphene quantum dots (GQDs) were conjectured to produce new or improve current methods used for bioimaging, drug delivery, and biomarker sensors for early detection of diseases. This review article critically compares and discusses current state-of-the-art use of GQDs in biology and health sciences. It shows the ability of GQDs to be easily functionalised for use as a targeted multimodal treatment and imaging platform. The in vitro and in vivo toxicity of GQDs are explored showing low toxicity for many types of GQDs.
Hyper-parallel photonic quantum computation with coupled quantum dots
Ren, Bao-Cang; Deng, Fu-Guo
2014-01-01
It is well known that a parallel quantum computer is more powerful than a classical one. So far, there are some important works about the construction of universal quantum logic gates, the key elements in quantum computation. However, they are focused on operating on one degree of freedom (DOF) of quantum systems. Here, we investigate the possibility of achieving scalable hyper-parallel quantum computation based on two DOFs of photon systems. We construct a deterministic hyper-controlled-not (hyper-CNOT) gate operating on both the spatial-mode and the polarization DOFs of a two-photon system simultaneously, by exploiting the giant optical circular birefringence induced by quantum-dot spins in double-sided optical microcavities as a result of cavity quantum electrodynamics (QED). This hyper-CNOT gate is implemented by manipulating the four qubits in the two DOFs of a two-photon system without auxiliary spatial modes or polarization modes. It reduces the operation time and the resources consumed in quantum information processing, and it is more robust against the photonic dissipation noise, compared with the integration of several cascaded CNOT gates in one DOF. PMID:24721781
Colloidal-quantum-dot spasers and plasmonic amplifiers
Kress, Stephan J P; Rohner, Patrik; Kim, David K; Antolinez, Felipe V; Zaininger, Karl-Augustin; Jayanti, Sriharsha V; Richner, Patrizia; McPeak, Kevin M; Poulikakos, Dimos; Norris, David J
2016-01-01
Colloidal quantum dots are robust, efficient, and tunable emitters now used in lighting, displays, and lasers. Consequently, when the spaser, a laser-like source of surface plasmons, was first proposed, quantum dots were specified as the ideal plasmonic gain medium. Subsequent spaser designs, however, have required a single material to simultaneously provide gain and define the plasmonic cavity, an approach ill-suited to quantum dots and other colloidal nanomaterials. Here we develop a more open architecture that decouples the gain medium from the cavity, leading to a versatile class of quantum-dot-based spasers that allow controlled generation, extraction, and manipulation of plasmons. We first create high-quality-factor, aberration-corrected, Ag plasmonic cavities. We then incorporate quantum dots via electrohydrodynamic printing18,19 or drop-casting. Photoexcitation under ambient conditions generates monochromatic plasmons above threshold. This signal is extracted, directed through an integrated amplifier,...
Non-blinking quantum dot with a plasmonic nanoshell resonator
Ji, Botao; Giovanelli, Emerson; Habert, Benjamin; Spinicelli, Piernicola; Nasilowski, Michel; Xu, Xiangzhen; Lequeux, Nicolas; Hugonin, Jean-Paul; Marquier, Francois; Greffet, Jean-Jacques; Dubertret, Benoit
2015-02-01
Colloidal semiconductor quantum dots are fluorescent nanocrystals exhibiting exceptional optical properties, but their emission intensity strongly depends on their charging state and local environment. This leads to blinking at the single-particle level or even complete fluorescence quenching, and limits the applications of quantum dots as fluorescent particles. Here, we show that a single quantum dot encapsulated in a silica shell coated with a continuous gold nanoshell provides a system with a stable and Poissonian emission at room temperature that is preserved regardless of drastic changes in the local environment. This novel hybrid quantum dot/silica/gold structure behaves as a plasmonic resonator with a strong Purcell factor, in very good agreement with simulations. The gold nanoshell also acts as a shield that protects the quantum dot fluorescence and enhances its resistance to high-power photoexcitation or high-energy electron beams. This plasmonic fluorescent resonator opens the way to a new family of plasmonic nanoemitters with robust optical properties.
Second-harmonic imaging of semiconductor quantum dots
DEFF Research Database (Denmark)
Østergaard, John Erland; Bozhevolnyi, Sergey I.; Pedersen, Kjeld;
2000-01-01
Resonant second-harmonic generation is observed at room temperature in reflection from self-assembled InAlGaAs quantum dots grown on a GaAs (001) substrate. The detected second-harmonic signal peaks at a pump wavelength of similar to 885 nm corresponding to the quantum-dot photoluminescence maximum....... In addition, the second-harmonic spectrum exhibits another smaller but well-pronounced peak at 765 nm not found in the linear experiments. We attribute this peak to the generation of second-harmonic radiation in the AlGaAs spacer layer enhanced by the local symmetry at the quantum-dot interface. We further...... observe that second-harmonic images of the quantum-dot surface structure show wavelength-dependent spatial variations. Imaging at different wavelength is used to demonstrate second-harmonic generation from the semiconductor quantum dots. (C) 2000 American Institute of Physics....
Quantum dots in diagnostics and detection: principles and paradigms.
Pisanic, T R; Zhang, Y; Wang, T H
2014-06-21
Quantum dots are semiconductor nanocrystals that exhibit exceptional optical and electrical behaviors not found in their bulk counterparts. Following seminal work in the development of water-soluble quantum dots in the late 1990's, researchers have sought to develop interesting and novel ways of exploiting the extraordinary properties of quantum dots for biomedical applications. Since that time, over 10,000 articles have been published related to the use of quantum dots in biomedicine, many of which regard their use in detection and diagnostic bioassays. This review presents a didactic overview of fundamental physical phenomena associated with quantum dots and paradigm examples of how these phenomena can and have been readily exploited for manifold uses in nanobiotechnology with a specific focus on their implementation in in vitro diagnostic assays and biodetection.
LUMINESCENCE OF CADMIUM SULFIDE QUANTUM DOTS IN FLUOROPHOSPHATE GLASSES
Directory of Open Access Journals (Sweden)
Z. O. Lipatova
2015-03-01
Full Text Available Cadmium sulfide quantum dots are perspective materials in optics, medicine, biology and optoelectronics. Fluorophosphate glasses, doped with cadmium sulfide quantum dots, were examined in the paper. Heat treatment led to the formation of quantum dots with diameters equal to 2.8 nm, 3.0 nm and 3.8 nm. In view of such changes in the quantum dots size the fundamental absorption edge shift and the luminescence band are being displaced to the long wavelengths. Luminescence lifetime has been found to be dependent on the registration wavelength in the range from 450 to 700 nm. Obtained fluorophosphate glasses with CdS quantum dots can find their application as fluorescent materials with intensive luminescence band and long excited-state natural lifetime.
Interaction of porphyrins with CdTe quantum dots
Energy Technology Data Exchange (ETDEWEB)
Zhang Xing; Liu Zhongxin; Ma Lun; Hossu, Marius; Chen Wei, E-mail: weichen@uta.edu [Department of Physics, University of Texas at Arlington, Box 19059 Arlington, TX 76019 (United States)
2011-05-13
Porphyrins may be used as photosensitizers for photodynamic therapy, photocatalysts for organic pollutant dissociation, agents for medical imaging and diagnostics, applications in luminescence and electronics. The detection of porphyrins is significantly important and here the interaction of protoporphyrin-IX (PPIX) with CdTe quantum dots was studied. It was observed that the luminescence of CdTe quantum dots was quenched dramatically in the presence of PPIX. When CdTe quantum dots were embedded into silica layers, almost no quenching by PPIX was observed. This indicates that PPIX may interact and alter CdTe quantum dots and thus quench their luminescence. The oxidation of the stabilizers such as thioglycolic acid (TGA) as well as the nanoparticles by the singlet oxygen generated from PPIX is most likely responsible for the luminescence quenching. The quenching of quantum dot luminescence by porphyrins may provide a new method for photosensitizer detection.
Self-assembled quantum dots in a nanowire system for quantum photonics
Heiss, M.; Fontana, Y.; Gustafsson, A; Wüst, G.; Magen, C.; O’Regan, D. D.; Luo, J. W.; Ketterer, B.; Conesa-Boj, S.; Kuhlmann, A. V.; Houel, J.; Russo-Averchi, E.; Morante, J. R.; Cantoni, M.; Marzari, N.
2013-01-01
Quantum dots embedded within nanowires represent one of the most promising technologies for applications in quantum photonics. Whereas the top-down fabrication of such structures remains a technological challenge, their bottom-up fabrication through self-assembly is a potentially more powerful strategy. However, present approaches often yield quantum dots with large optical linewidths, making reproducibility of their physical properties difficult. We present a versatile quantum-dot-innanowire...
Templated self-assembly of SiGe quantum dots
Energy Technology Data Exchange (ETDEWEB)
Dais, Christian
2009-08-19
This PhD thesis reports on the fabrication and characterization of exact aligned SiGe quantum dot structures. In general, SiGe quantum dots which nucleate via the Stranski-Krastanov growth mode exhibit broad size dispersion and nucleate randomly on the surface. However, to tap the full potential of SiGe quantum dots it is necessary to control the positioning and size of the dots on a nanometer length, e.g. for electronically addressing of individual dots. This can be realized by so-called templated self-assembly, which combines top-down lithography with bottom-up selfassembly. In this process the lithographically defined pits serve as pre-defined nucleation points for the epitaxially grown quantum dots. In this thesis, extreme ultraviolet interference lithography at a wavelength of e=13.4 nm is employed for prepatterning of the Si substrates. This technique allows the precise and fast fabrication of high-resolution templates with a high degree of reproducibility. The subsequent epitaxial deposition is either performed by molecular beam epitaxy or low-pressure chemical vapour deposition. It is shown that the dot nucleation on pre-patterned substrates depends strongly on the lithography parameters, e.g. size and periodicity of the pits, as well as on the epitaxy parameters, e.g. growth temperature or material coverage. The interrelations are carefully analyzed by means of scanning force microscopy, transmission electron microscopy and X-ray diffraction measurements. Provided that correct template and overgrowth parameters are chosen, perfectly aligned and uniform SiGe quantum dot arrays of different period, size as well as symmetry are created. In particular, the quantum dot arrays with the so far smallest period (35 nm) and smallest size dispersion are fabricated in this thesis. Furthermore, the strain fields of the underlying quantum dots allow the fabrication of vertically aligned quantum dot stacks. Combining lateral and vertical dot alignment results in three
The Electron－Hole Pair in a Single Quantum Dot and That in a Vertically Coupled Quantum Dot
Institute of Scientific and Technical Information of China (English)
XIEWen-Fang; ZHUWu
2003-01-01
The energy spectra of low-lying states of an exciton in a single and a vertically coupled quantum dots are studied under the influence of a perpendicularly applied magnetic field. Calculations are made by using the method of numerical diagonalization of the Hamiltonian within the effective-mass approximation. We also calculated the binding energy of the ground and the excited states of an exciton in a single quantum dot and that in a vertically coupled quantum dot as a function of the dot radius for different vaJues of the distance and the magnetic field strength.
Schreiber, K. A.; Samkharadze, N.; Gardner, G. C.; Biswas, Rudro R.; Manfra, M. J.; Csáthy, G. A.
2017-07-01
Under hydrostatic pressure, the ground state of a two-dimensional electron gas at ν =5 /2 changes from a fractional quantum Hall state to the stripe phase. By measuring the energy gap of the fractional quantum Hall state and of the onset temperature of the stripe phase, we mapped out a phase diagram of these competing phases in the pressure-temperature plane. Our data highlight the dichotomy of two descriptions of the half-filled Landau level near the quantum critical point: one based on electrons and another on composite fermions.
Biosensing with Luminescent Semiconductor Quantum Dots
Directory of Open Access Journals (Sweden)
Hedi Mattoussi
2006-08-01
Full Text Available Luminescent semiconductor nanocrystals or quantum dots (QDs are a recentlydeveloped class of nanomaterial whose unique photophysical properties are helping tocreate a new generation of robust fluorescent biosensors. QD properties of interest forbiosensing include high quantum yields, broad absorption spectra coupled to narrow sizetunablephotoluminescent emissions and exceptional resistance to both photobleaching andchemical degradation. In this review, we examine the progress in adapting QDs for severalpredominantly in vitro biosensing applications including use in immunoassays, asgeneralized probes, in nucleic acid detection and fluorescence resonance energy transfer(FRET - based sensing. We also describe several important considerations when workingwith QDs mainly centered on the choice of material(s and appropriate strategies forattaching biomolecules to the QDs.
Semiconductor Quantum Dots for Biomedicial Applications
Shao, Lijia; Gao, Yanfang; Yan, Feng
2011-01-01
Semiconductor quantum dots (QDs) are nanometre-scale crystals, which have unique photophysical properties, such as size-dependent optical properties, high fluorescence quantum yields, and excellent stability against photobleaching. These properties enable QDs as the promising optical labels for the biological applications, such as multiplexed analysis of immunocomplexes or DNA hybridization processes, cell sorting and tracing, in vivo imaging and diagnostics in biomedicine. Meanwhile, QDs can be used as labels for the electrochemical detection of DNA or proteins. This article reviews the synthesis and toxicity of QDs and their optical and electrochemical bioanalytical applications. Especially the application of QDs in biomedicine such as delivering, cell targeting and imaging for cancer research, and in vivo photodynamic therapy (PDT) of cancer are briefly discussed. PMID:22247690
Semiconductor quantum dot-sensitized solar cells.
Tian, Jianjun; Cao, Guozhong
2013-10-31
Semiconductor quantum dots (QDs) have been drawing great attention recently as a material for solar energy conversion due to their versatile optical and electrical properties. The QD-sensitized solar cell (QDSC) is one of the burgeoning semiconductor QD solar cells that shows promising developments for the next generation of solar cells. This article focuses on recent developments in QDSCs, including 1) the effect of quantum confinement on QDSCs, 2) the multiple exciton generation (MEG) of QDs, 3) fabrication methods of QDs, and 4) nanocrystalline photoelectrodes for solar cells. We also make suggestions for future research on QDSCs. Although the efficiency of QDSCs is still low, we think there will be major breakthroughs in developing QDSCs in the future.
Semiconductor quantum dot-sensitized solar cells
Directory of Open Access Journals (Sweden)
Jianjun Tian
2013-10-01
Full Text Available Semiconductor quantum dots (QDs have been drawing great attention recently as a material for solar energy conversion due to their versatile optical and electrical properties. The QD-sensitized solar cell (QDSC is one of the burgeoning semiconductor QD solar cells that shows promising developments for the next generation of solar cells. This article focuses on recent developments in QDSCs, including 1 the effect of quantum confinement on QDSCs, 2 the multiple exciton generation (MEG of QDs, 3 fabrication methods of QDs, and 4 nanocrystalline photoelectrodes for solar cells. We also make suggestions for future research on QDSCs. Although the efficiency of QDSCs is still low, we think there will be major breakthroughs in developing QDSCs in the future.
Electron states in semiconductor quantum dots
Energy Technology Data Exchange (ETDEWEB)
Dhayal, Suman S., E-mail: ssdhayal@gmail.com [Department of Physics, University of North Texas, P.O. Box 311427, Denton, Texas 76203 (United States); Ramaniah, Lavanya M., E-mail: lavanya@barc.gov.in [High Pressure and Synchrotron Radiation Physics Division, Physics Group, Bhabha Atomic Research Centre, Trombay, Mumbai 400085 (India); Ruda, Harry E.; Nair, Selvakumar V., E-mail: selva.nair@utoronto.ca [Centre for Nanotechnology, University of Toronto, 170 College Street, Toronto, Ontario M5S 3E3 (Canada)
2014-11-28
In this work, the electronic structures of quantum dots (QDs) of nine direct band gap semiconductor materials belonging to the group II-VI and III-V families are investigated, within the empirical tight-binding framework, in the effective bond orbital model. This methodology is shown to accurately describe these systems, yielding, at the same time, qualitative insights into their electronic properties. Various features of the bulk band structure such as band-gaps, band curvature, and band widths around symmetry points affect the quantum confinement of electrons and holes. These effects are identified and quantified. A comparison with experimental data yields good agreement with the calculations. These theoretical results would help quantify the optical response of QDs of these materials and provide useful input for applications.