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Sample records for surface spin excitations

  1. Spin-polarized spin excitation spectroscopy

    Energy Technology Data Exchange (ETDEWEB)

    Loth, Sebastian; Lutz, Christopher P; Heinrich, Andreas J, E-mail: lothseb@us.ibm.com, E-mail: heinrich@almaden.ibm.com [IBM Research Division, Almaden Research Center, San Jose, CA 95120 (United States)

    2010-12-15

    We report on the spin dependence of elastic and inelastic electron tunneling through transition metal atoms. Mn, Fe and Cu atoms were deposited onto a monolayer of Cu{sub 2}N on Cu(100) and individually addressed with the probe tip of a scanning tunneling microscope. Electrons tunneling between the tip and the substrate exchange energy and spin angular momentum with the surface-bound magnetic atoms. The conservation of energy during the tunneling process results in a distinct onset threshold voltage above which the tunneling electrons create spin excitations in the Mn and Fe atoms. Here we show that the additional conservation of spin angular momentum leads to different cross-sections for spin excitations depending on the relative alignment of the surface spin and the spin of the tunneling electron. For this purpose, we developed a technique for measuring the same local spin with a spin-polarized and a non-spin-polarized tip by exchanging the last apex atom of the probe tip between different transition metal atoms. We derive a quantitative model describing the observed excitation cross-sections on the basis of an exchange scattering process.

  2. Localized excitation of magnetostatic surface spin waves in yttrium iron garnet by shorted coaxial probe detected via spin pumping and rectification effect

    Energy Technology Data Exchange (ETDEWEB)

    Soh, Wee Tee, E-mail: a0046479@u.nus.edu; Ong, C. K. [Center for Superconducting and Magnetic Materials, Department of Physics, National University of Singapore, 2 Science Drive 3, Singapore 117551 (Singapore); Peng, Bin [State Key Laboratory of Electronic Thin Films and Integrated Devices, University of Electronic Science and Technology of China, Chengdu 610054 (China)

    2015-04-21

    We demonstrate the localized excitation and dc electrical detection of magnetostatic surface spin waves (MSSWs) in yttrium iron garnet (YIG) by a shorted coaxial probe. Thin films of NiFe and Pt are patterned at different regions onto a common bulk YIG substrate. A shorted coaxial probe is used to excite spin precession locally near various patterned regions. The dc voltages across the corresponding regions are recorded. For excitation of the Pt regions, the dc voltage spectra are dominated by the spin pumping of MSSWs from YIG, where various modes can be clearly distinguished. For the NiFe region, it is also found that spin pumping from MSSWs generated in YIG dominated the spectra, indicating that the spin pumped currents are dissipated into charge currents via the inverse Spin Hall effect (ISHE) in NiFe. For all regions, dc signals from YIG MSSWs are observed to be much stronger than the ferromagnetic resonance (FMR) uniform mode, likely due to the nature of the microwave excitation. The results indicate the potential of this probe for microwave imaging via dc detection of spin dynamics in continuous and patterned films.

  3. Effect of Fermi surface nesting on resonant spin excitations in Ba(1-x)K(x)Fe2As2.

    Science.gov (United States)

    Castellan, J-P; Rosenkranz, S; Goremychkin, E A; Chung, D Y; Todorov, I S; Kanatzidis, M G; Eremin, I; Knolle, J; Chubukov, A V; Maiti, S; Norman, M R; Weber, F; Claus, H; Guidi, T; Bewley, R I; Osborn, R

    2011-10-21

    We report inelastic neutron scattering measurements of the resonant spin excitations in Ba(1-x)K(x)Fe(2)As(2) over a broad range of electron band filling. The fall in the superconducting transition temperature with hole doping coincides with the magnetic excitations splitting into two incommensurate peaks because of the growing mismatch in the hole and electron Fermi surface volumes, as confirmed by a tight-binding model with s(±)-symmetry pairing. The reduction in Fermi surface nesting is accompanied by a collapse of the resonance binding energy and its spectral weight, caused by the weakening of electron-electron correlations.

  4. Effect of Fermi surface nesting on resonant spin excitations in Ba{<_1-x}K{<_x}Fe{<_2}As{<_2}.

    Energy Technology Data Exchange (ETDEWEB)

    Castellan, J.-P.; Rosenkranz, S.; Goremychkin, E.A.; Chung, D.Y.; Todorov, I.S.; Kanatzidis, M.G.; Eremin, I.; Knolle, J.; Chubukov, A.V.; Maiti, s.; Norman, M.R.; Weber, F.; Claus, H.; Guidi, T.; Bewley, R.I.; Osborn, R. (Materials Science Division); (Northwestern Univ.); (Ruhr Univ.); (Max-Planck-Institut fur Physik komplexer Systeme); (Univ. Wisconsin-Madison); (Rutherford AppletonLab)

    2011-01-01

    We report inelastic neutron scattering measurements of the resonant spin excitations in Ba{sub 1-x}K{sub x}Fe{sub 2}As{sub 2} over a broad range of electron band filling. The fall in the superconducting transition temperature with hole doping coincides with the magnetic excitations splitting into two incommensurate peaks because of the growing mismatch in the hole and electron Fermi surface volumes, as confirmed by a tight-binding model with s{sub {+-}}-symmetry pairing. The reduction in Fermi surface nesting is accompanied by a collapse of the resonance binding energy and its spectral weight, caused by the weakening of electron-electron correlations.

  5. Spin Transport by Collective Spin Excitations

    Science.gov (United States)

    Hammel, P. Chris

    We report studies of angular momentum transport in insulating materials. Our measurements reveal efficient spin pumping from high wavevector k spin waves in thin film Y3Fe5O12 (YIG): spin pumping is independent of wavevector up to k ~ 20 μm-1. Optical detection of YIG FMR by NV centers in diamond reveals a role for spin waves in this insulator-to-insulator spin transfer process. Spin transport is typically suppressed by insulating barriers, but we find that fluctuating antiferromagnetic correlations enable efficient spin transport at nm-scale thicknesses in insulating antiferromagnets, even in the absence of long-range order, and that the spin decay length increases with the strength of the antiferromagnetic correlations. This research is supported by the U.S. DOE through Grants DE-FG02-03ER46054 and DE-SC0001304, by the NSF MRSEC program through Grant No. 1420451 and by the Army Research Office through Grant W911NF0910147.

  6. Spin-wave multiple excitations in nanoscale classical Heisenberg antiferromagnets

    Energy Technology Data Exchange (ETDEWEB)

    Hou, Zhuofei [University of Georgia, Athens; Landau, David P [University of Georgia, Athens; Stocks, George Malcolm [ORNL; Brown, G. [Florida State University, Tallahassee

    2015-02-17

    Monte Carlo and spin dynamics techniques have been used to perform large-scale simulations of the dynamic behavior of a nanoscale, classical, Heisenberg antiferromagnet on a simple-cubic lattice with linear sizes L≤ 40 at a temperature below the Neel temperature. In this study, nanoparticles are modeled with completely free boundary conditions, i.e., six free surfaces, and nanofilms are modeled with two free surfaces in the spatial z direction and periodic boundaries parallel to the surfaces in the xy direction, which are compared to the infinite system with periodic boundary conditions. The temporal evolutions of spin configurations were determined numerically from coupled equations of motion for individual spins using a fast spin dynamics algorithm with the fourth-order Suzuki-Trotter decomposition of exponential operators, with initial spin configurations generated by Monte Carlo simulations. The local dynamic structure factor S(q,ω) was calculated from the local space- and time-displaced spin-spin correlation function. Multiple excitation peaks for wave vectors within the first Brillouin zone appear in the spin-wave spectra of the transverse component of dynamic structure factor ST (q,ω) in the nanoscale classical Heisenberg antiferromagnet, which are lacking if periodic boundary conditions are used. With the assumption of q-space spin-wave reflections with broken momentum conservation due to free-surface confinements, we successfully explained those spectra quantitatively in the linear dispersion region. Meanwhile, we also observed two unexpected quantized spin-wave excitation modes in the spatial z direction in nanofilms for ST (q,ω) not expected in bulk systems. In conclusion, the results of this study indicate the presence of unexpected forms of spin-wave excitation behavior that have yet to be observed experimentally but could be directly tested through neutron scattering experiments on nanoscale RbMnF3 particles or

  7. Spin-orbit coupling in the dissociative excitation of alkali atoms at the surface of rare gas clusters: A theoretical study.

    Science.gov (United States)

    Gervais, B; Zanuttini, D; Douady, J

    2016-05-21

    We analyze the role of the spin-orbit (SO) coupling in the dissociative dynamics of excited alkali atoms at the surface of small rare gas clusters. The electronic structure of the whole system is deduced from a one-electron model based on core polarization pseudo-potentials. It allows us to obtain in the same footing the energy, forces, and non-adiabatic couplings used to simulate the dynamics by means of a surface hopping method. The fine structure state population is analyzed by considering the relative magnitude of the SO coupling ξ, with respect to the spin-free potential energy. We identify three regimes of ξ-values leading to different evolution of adiabatic state population after excitation of the system in the uppermost state of the lowest np (2)P shell. For sufficiently small ξ, the final population of the J=12 atomic states, P12, grows up linearly from P12=13 at ξ = 0 after a diabatic dynamics. For large values of ξ, we observe a rather adiabatic dynamics with P12 decreasing as ξ increases. For intermediate values of ξ, the coupling is extremely efficient and a complete transfer of population is observed for the set of parameters associated to NaAr3 and NaAr4 clusters.

  8. Topological Excitations in Quantum Spin Systems

    Directory of Open Access Journals (Sweden)

    Ranjan Chaudhury

    2013-01-01

    Full Text Available The origin and significance of topological excitations in quantum spin models in low dimensions are presented in detail. Besides a general review, our own work in this area is described in great depth. Apart from theoretical analysis of the existence and properties of spin vortices and antivortices, the possible experimental consequences and signatures are also highlighted. In particular, the distinguishing features between the even and odd charged topological excitations are brought out through a detailed analysis of the topological term in the quantum action. Moreover, an interesting symmetry property is predicted between the excitations from a ferromagnetic model and an antiferromagnetic model. Through a novel approach of ours, a bridge is established between field theoretical formalism and the well-known statistical mechanical treatment of Berezinskii-Kosterlitz-Thouless (BKT transition involving these topological excitations. Furthermore, a detailed phenomenological analysis of the experimentally observed static and dynamic magnetic properties of the layered magnetic materials, possessing XY anisotropy in the in-plane spin-spin couplings, is undertaken to test the theoretical predictions regarding the behaviour of these excitations. The importance and the crucial role of quantum spin fluctuations in these studies are also brought out very clearly by our analysis.

  9. Spin Excitations in Dissipative Ferromagnetic Nanoshells

    Directory of Open Access Journals (Sweden)

    V.V. Kulish

    2016-10-01

    Full Text Available In the paper, dipole-exchange radial-angular spin excitations in a spherical ferromagnetic nanoshell are investigated. For such excitations, a differential equation for the magnetic potential is found, with account for the magnetic dipole-dipole interaction, the exchange interaction, the anisotropy effects and the dissipation. The equation is solved for the three cases – the case of a thin shell, the case of short waves and the case of radial excitations. For each of these cases, the dispersion relation and the spectrum of possible excitation frequencies are found.

  10. Spin-flip, tensor equation-of-motion configuration interaction with a density-functional correction: A spin-complete method for exploring excited-state potential energy surfaces

    Science.gov (United States)

    Zhang, Xing; Herbert, John M.

    2015-12-01

    We revisit the formalism of the spin-adapted, spin-flip (SA-SF) configuration-interaction singles (CIS) method based on a tensor equation-of-motion formalism that affords proper spin eigenstates without sacrificing single-reference simplicity. Matrix elements for SA-SF-CIS are then modified in a manner similar to collinear spin-flip time-dependent density functional theory (SF-TDDFT), to include a DFT exchange-correlation correction. The performance of this method, which we call SA-SF-DFT, is evaluated numerically and we find that it systematically improves the energies of electronic states that exhibit significant spin contamination within the conventional SF-TDDFT approach. The new method cures the state assignment problem that plagues geometry optimizations and ab initio molecular dynamics simulations using traditional SF-TDDFT, without sacrificing computational efficiency, and furthermore provides correct topology at conical intersections, including those that involve the ground state, unlike conventional TDDFT. As such, SA-SF-DFT appears to be a promising method for generating excited-state potential energy surfaces at DFT cost.

  11. Edge Magnon Excitation in Spin Dimer Systems

    Science.gov (United States)

    Sakaguchi, Ryo; Matsumoto, Masashige

    2016-10-01

    Magnetic excitation in a spin dimer system on a bilayer honeycomb lattice is investigated in the presence of a zigzag edge, where disordered and ordered phases can be controlled by a quantum phase transition. In analogy with the case of graphene with a zigzag edge, a flat edge magnon mode appears in the disordered phase. In an ordered phase, a finite magnetic moment generates a mean-field potential to the magnon. Since the potential is nonuniform on the edge and bulk sites, it affects the excitation, and the dispersion of the edge mode deviates from the flat shape. We investigate how the edge magnon mode evolves when the phase changes through the quantum phase transition and discuss the similarities to ordered spin systems on a monolayer honeycomb lattice.

  12. Spin voltage generation through optical excitation of complementary spin populations

    Science.gov (United States)

    Bottegoni, Federico; Celebrano, Michele; Bollani, Monica; Biagioni, Paolo; Isella, Giovanni; Ciccacci, Franco; Finazzi, Marco

    2014-08-01

    By exploiting the spin degree of freedom of carriers inside electronic devices, spintronics has a huge potential for quantum computation and dissipationless interconnects. Pure spin currents in spintronic devices should be driven by a spin voltage generator, able to drive the spin distribution out of equilibrium without inducing charge currents. Ideally, such a generator should operate at room temperature, be highly integrable with existing semiconductor technology, and not interfere with other spintronic building blocks that make use of ferromagnetic materials. Here we demonstrate a device that matches these requirements by realizing the spintronic equivalent of a photovoltaic generator. Whereas a photovoltaic generator spatially separates photoexcited electrons and holes, our device exploits circularly polarized light to produce two spatially well-defined electron populations with opposite in-plane spin projections. This is achieved by modulating the phase and amplitude of the light wavefronts entering a semiconductor (germanium) with a patterned metal overlayer (platinum). The resulting light diffraction pattern features a spatially modulated chirality inside the semiconductor, which locally excites spin-polarized electrons thanks to electric dipole selection rules.

  13. Detecting spin fractionalization in a spinon Fermi surface spin liquid

    Science.gov (United States)

    Li, Yao-Dong; Chen, Gang

    2017-08-01

    Motivated by the recent proposal that several candidate materials such as YbMgGaO4 could be spinon Fermi surface spin liquids, we explore the experimental consequences of the external magnetic fields on this exotic state. Specifically, we focus on the weak field regime where the spin-liquid state is well preserved and the spinon remains to be a good description of the magnetic excitations. From the spin-1/2 nature of the spinon excitation, we predict the unique features of the spinon continuum when the weak magnetic field is applied to the system. Due to the small energy scale of the exchange interactions between the local moments in the spin-liquid candidate like YbMgGaO4, our proposal for the spectral weight shifts and spectral crossing in the magnetic fields can be immediately tested by inelastic neutron scattering experiments. Several other experimental aspects about the spinon Fermi surface and the spinon excitations are discussed and proposed. Our work provides an experimental scheme to examine the fractionalized spinon excitation and the candidate spin-liquid states in YbMgGaO4, the 6H-B phase of Ba3NiSb2O9 , and other relevant materials.

  14. Spin-flavor composition of excited baryons

    Science.gov (United States)

    Fernando, Ishara; Goity, Jose

    2015-10-01

    The excited baryon masses are analyzed in the framework of the 1 /Nc expansion using the available physical masses and also the masses obtained in lattice QCD for different quark masses. The baryon states are organized into irreducible representations of SU (6) × O (3) , where the [ 56 ,lP =0+ ] ground state and excited baryons, and the [ 56 ,2+ ] and [ 70 ,1- ] excited states are analyzed. The analyses are carried out to O 1 /Nc and first order in the quark masses. The issue of state identifications is discussed. Numerous parameter independent mass relations result at those orders, among them the well known Gell-Mann-Okubo and Equal Spacing relations, as well as additional relations involving baryons with different spins. It is observed that such relations are satisfied at the expected level of precision. Predictions for physically unknown states for each multiplet are obtained. From the quark-mass dependence of the coefficients in the baryon mass formulas an increasingly simpler picture of the spin-flavor composition of the baryons is observed with increasing pion mass (equivalently, increasing mu , d masses), as measured by the number of significant mass operators. This work was supported in part by DOE Contract No. DE-AC05-06OR23177 under which JSA operates the Thomas Jefferson National Accelerator Facility (J. L. G.), and by the NSF (USA) through Grant PHY-0855789 and PHY-1307413 (I. P. F and J. L. G).

  15. Excited-State Spectroscopy Using Single Spin Manipulation in Diamond

    NARCIS (Netherlands)

    Fuchs, G.D.; Dobrovitski, V.V.; Hanson, R.; Batra, A.; Weis, C.D.; Schenkel, T.; Awschalom, D.D.

    2008-01-01

    We use single-spin resonant spectroscopy to study the spin structure in the orbital excited state of a diamond nitrogen-vacancy (N-V) center at room temperature. The data show that the excited-state spin levels have a zero-field splitting that is approximately half of the value of the ground state

  16. Superdirected Beam of the Surface Spin Wave

    CERN Document Server

    Annenkov, Alexander Yu; Lock, Edwin H

    2016-01-01

    Visualized diffraction patterns of the surface spin wave excited by arbitrarily oriented linear transducer in tangentially magnetized ferrite film are investigated experimentally in the plane of ferrite film for the case where the transducer length D is much larger than the wavelength L. Superdirected (nonexpanding) beam of the surface spin wave with noncollinear wave vector k and group velocity vector V was observed experimentally: the angular width of this beam was about zero, the smearing of the beam energy along the film plane was minimal and the length of the beam trajectory was maximal (50 mm). Thus it was shown that such phenomenon as superdirected propagation of the wave exists in the nature.

  17. Transverse Chiral Optical Forces by Locally Excited Surface Plasmon Polaritons

    CERN Document Server

    Alizadeh, M H

    2015-01-01

    Recently the new concepts of transverse spin angular momentum and Belinfante spin momentum of evanescent waves have drawn considerable attention. Here, we investigate these novel physical properties of electromagnetic fields in the context of locally excited surface plasmon polaritons. We demonstrate, both analytically and numerically, that locally excited surface plasmon polaritons possess transverse spin angular momentum and Belinfante momentum with rich and non-trivial characteristics. We also show that the transverse spin angular momentum of locally excited surface plasmon polaritons leads to the emergence of transverse chiral forces in opposite directions for chiral objects of different handedness. The magnitude of such a transverse force is comparable to the optical gradient force and scattering forces. This finding may pave the way for realization of optical separation of chiral biomolecules.

  18. Squeezing of Collective Excitations in Spin Ensembles

    DEFF Research Database (Denmark)

    Kraglund Andersen, Christian; Mølmer, Klaus

    2012-01-01

    We analyse the possibility to create two-mode spin squeezed states of two separate spin ensembles by inverting the spins in one ensemble and allowing spin exchange between the ensembles via a near resonant cavity field. We investigate the dynamics of the system using a combination of numerical an...

  19. Excitation of spin echo by pulses with linear frequency modulation

    Science.gov (United States)

    Baruzdin, S. A.

    2015-03-01

    The excitation of a spin echo by two pulses with linear frequency modulation, upon which the pulse parameters ensure maximal compression of the response in time, is considered. The frequency of the excitation pulses was changed by a step law, approximating its linear rise. The transfer matrix of the state of the spin system for pulses with linear frequency modulation is found by solving the Bloch equations. The shape of the envelope of the spin echo in thin magnetic cobalt films, as well as the dependence of the echo amplitude on the parameters of the excitation pulses, is determined. The amplitudes of the excitation pulses, which ensure the excitation of the echo maximal amplitude for various values of the frequency deviation, are found. It is shown that the use of pulses with linear frequency modulation makes it possible to obtain the same echo amplitude as with the use of simple excitation pulses for a substantially smaller amplitude and power of excitation pulses.

  20. Surface spin-valve effect.

    Science.gov (United States)

    Yanson, I K; Naidyuk, Yu G; Fisun, V V; Konovalenko, A; Balkashin, O P; Triputen, L Yu; Korenivski, V

    2007-04-01

    We report an observation of spin-valve-like hysteresis within a few atomic layers at a ferromagnetic interface. We use phonon spectroscopy of nanometer-sized point contacts as an in situ probe to study the mechanism of the effect. Distinctive energy phonon peaks for contacts with dissimilar nonmagnetic outer electrodes allow localizing the observed spin switching to the top or bottom interfaces for nanometer thin ferromagnetic layers. The mechanism consistent with our data is energetically distinct atomically thin surface spin layers that can form current- or field-driven surface spin-valves within a single ferromagnetic film.

  1. Angular dependent study on ferromagnetic resonance and spin excitations by spin rectification

    Energy Technology Data Exchange (ETDEWEB)

    Zhang, Yichao; Fan, Xiaolong, E-mail: fanxiaolong@lzu.edu.cn; Zhao, Xiaobing; Rao, Jinwei; Zhou, Hengan; Guo, Dangwei; Xue, Desheng [The Key Lab for Magnetism and Magnetic Materials of Ministry of Education, Lanzhou University, Lanzhou 730000 (China); Gui, Y. S.; Hu, C.-M. [Department of Physics and Astronomy, University of Manitoba, Winnipeg, Manitoba R3T 2N2 (Canada)

    2015-01-14

    We report angular dependent spin rectification spectra which are applied to studying spin excitations in single permalloy stripe. Based on planar Hall effect, those spin excitations generate special resonant dc Hall voltages, which have been characterized as functions of the amplitude and direction of applied magnetic field. Through high angular resolution 2D mappings, the evolutions of different spin excitation can be directly presented, and the dynamic magnetic parameters such as the gyromagnetic ratio, effective exchange field, as well as the quantized numbers of standing spin waves can be accurately determined through fitting the angular evolution of each resonance.

  2. From spin flip excitations to the spin susceptibility enhancement of a two-dimensional electron gas.

    Science.gov (United States)

    Perez, F; Aku-leh, C; Richards, D; Jusserand, B; Smith, L C; Wolverson, D; Karczewski, G

    2007-07-13

    The g-factor enhancement of the spin-polarized two-dimensional electron gas was measured directly over a wide range of spin polarizations, using spin flip resonant Raman scattering spectroscopy on two-dimensional electron gases embedded in Cd(1-x)Mn(x)Te semimagnetic quantum wells. At zero Raman transferred momentum, the single-particle spin flip excitation, energy Z*, coexists in the Raman spectrum with the spin flip wave of energy Z, the bare giant Zeeman splitting. We compare the measured g-factor enhancement with recent spin-susceptibility enhancement theories and deduce the spin-polarization dependence of the mass renormalization.

  3. Nonlinear spin-wave excitations at low magnetic bias fields

    Science.gov (United States)

    Woltersdorf, Georg

    We investigate experimentally and theoretically the nonlinear magnetization dynamics in magnetic films at low magnetic bias fields. Nonlinear magnetization dynamics is essential for the operation of numerous spintronic devices ranging from magnetic memory to spin torque microwave generators. Examples are microwave-assisted switching of magnetic structures and the generation of spin currents at low bias fields by high-amplitude ferromagnetic resonance. In the experiments we use X-ray magnetic circular dichroism to determine the number density of excited magnons in magnetically soft Ni80Fe20 thin films. Our data show that the common Suhl instability model of nonlinear ferromagnetic resonance is not adequate for the description of the nonlinear behavior in the low magnetic field limit. Here we derive a model of parametric spin-wave excitation, which correctly predicts nonlinear threshold amplitudes and decay rates at high and at low magnetic bias fields. In fact, a series of critical spin-wave modes with fast oscillations of the amplitude and phase is found, generalizing the theory of parametric spin-wave excitation to large modulation amplitudes. For these modes, we also find pronounced frequency locking effects that may be used for synchronization purposes in magnonic devices. By using this effect, effective spin-wave sources based on parametric spin-wave excitation may be realized. Our results also show that it is not required to invoke a wave vector-dependent damping parameter in the interpretation of nonlinear magnetic resonance experiments performed at low bias fields.

  4. Skyrmions and edge-spin excitations in quantum Hall droplets

    Energy Technology Data Exchange (ETDEWEB)

    Oaknin, J.H. [Departamento de Fisica Teorica de la Materia Condensada, Universidad Autonoma de Madrid, Cantoblanco, 28049, Madrid (Spain); Martin-Moreno, L. [Departamento de Fisica de la Materia Condensada, Instituto de Ciencia de Materiales de Aragon, Consejo Superior de Investigaciones Cientificas, Universidad de Zaragoza, Zaragoza 50015 (Spain); Tejedor, C. [Departamento de Fisica Teorica de la Materia Condensada, Universidad Autonoma de Madrid, Cantoblanco, 28049, Madrid (Spain)

    1996-12-01

    We present a microscopic analysis of spin textures in quantum Hall droplets for filling factors {nu}{approx_equal}1. We obtain analytical many-body wave functions of spin excitations which describe all of the necessary quantum numbers. An adequate linear combination of these eigenstates leads to wave functions in which the spatially dependent spinor can be factorized. This displays the topological structure of several spin textures, some of which are located at the bulk, and others at the edge. For the former, we obtain bulk charged skyrmions that can be expressed as a condensate of spin excitons interacting via a two-body repulsive interaction. The size of the skyrmion is given by the number of excitons present in the condensate. We also obtain the skyrmion energy as a function of its size for both zero and finite Zeeman energy. For the edge excitations we find that a branch of these spin textures starts with lower energy than the branch of polarized charge edge excitations. When the number of electrons is of the order of a few tenths, there are no crossings of the spin and charge branches so that edge-spin textures can be responsible for the edge reconstruction of the droplet. On the contrary, edge reconstruction is always found to be due to polarized charge excitations when the number of electrons is larger than one hundred. {copyright} {ital 1996 The American Physical Society.}

  5. Excitation of plasmons in Ag/Fe/W structure by spin-polarized electrons

    Energy Technology Data Exchange (ETDEWEB)

    Samarin, Sergey N.; Kostylev, Mikhail; Williams, J. F. [School of Physics, The University of Western Australia, Perth WA 6009 (Australia); Artamonov, Oleg M.; Baraban, Alexander P. [St. Petersburg State University, Faculty of Physics, St. Petersburg 199034 (Russian Federation); Guagliardo, Paul [Centre for Microscopy, Characterisation and Analysis, The University of Western Australia, Perth WA 6009 (Australia)

    2015-09-07

    Using Spin-polarized Electron-Energy Loss Spectroscopy (SPEELS), the plasmon excitations were probed in a few atomic layers thick Ag film deposited on an Fe layer or on a single crystal of W(110). The measurements were performed at two specular geometries with either a 25° or 72° angle of incidence. On a clean Fe layer (10 atomic layers thick), Stoner excitation asymmetry was observed, as expected. Deposition of a silver film on top of the Fe layer dramatically changed the asymmetry of the SPEELS spectra. The spin-effect depends on the kinematics of the scattering: angles of incidence and detection. The spin-dependence of the plasmon excitations in the silver film on the W(110) surface and on the ferromagnetic Fe film is suggested to arise from the spin-active Ag/W or Ag/Fe interfaces.

  6. Theory of spin excitations in Fe(110) monolayers

    Science.gov (United States)

    Muniz, R. B.; Mills, D. L.

    2002-11-01

    We present theoretical studies of short-wavelength spin excitations in ferromagnetic Fe(110) monolayers either adsorbed on a W(110) substrate or free standing. We use an itinerant model of electrons as the basis for our analysis, with nine bands (the five 3d bands and the 4sp complex) included. The bands are described within an empirical tight-binding scheme, and the ferromagnetic ground state is generated from on-site intraatomic Coulomb interactions, described in mean-field theory. The random phase approximation (RPA) is employed to describe the spin excitations through analysis of the wave vector and frequency dependence of the dynamic transverse susceptibility. Several issues are explored. We compare the spin-wave stiffness and other features of the spin-wave spectrum for the free standing film and that adsorbed on the substrate to find substantial quantitative differences with origin in spin-spin interactions mediated by the substrate. We also compare the spin-wave spectrum calculated through use of the RPA, an approximate theory, but a scheme that does not invoke the adiabatic approximation, with results generated within the framework of the adiabatic approach. While the spin-wave exchange stiffnesses produced by the two methods are in agreement, there are substantial differences between excitation spectra at short wavelengths. We argue that effective interspin exchange couplings generated within the framework of the adiabatic approximation fail to provide a description of the spin-wave spectrum in the itinerant ferromagnets, beyond the low-frequency, long-wavelength regime where the spin-wave exchange stiffness suffices to describe the spectrum. We also discuss apparent hybridization gaps in the spin-wave spectrum. We show that in some cases they can be artifact of a poorly converged numerical analysis and, in one instance, on use of an inappropriate form for the intra-atomic Coulomb interaction.

  7. Thermally excited magnonic spin currents probed by the longitudinal spin-Seebeck effect in YIG

    Energy Technology Data Exchange (ETDEWEB)

    Kehlberger, Andreas; Roeser, Rene; Jakob, Gerhard; Klaeui, Mathias [Institute of Physics, Johannes Gutenberg-University Mainz, 55099 Mainz (Germany); Jungfleisch, Benjamin; Hillebrands, Burkard; Nowak, Ulrich [Department of Physics, Institute of Technology Kaiserslautern, 67663 Kaiserslautern (Germany); Ritzmann, Ulrike; Hinzke, Denise [Department of Physics, University of Konstanz, 78457 Konstanz (Germany); Kim, Dong Hun; Ross, Caroline [Department of Materials Science and Engineering, MIT, Cambridge, MA 02139 (United States)

    2013-07-01

    In the research field of spin caloric transport one of most the prominent and still not understood effects is the spin-Seebeck effect (SSE) in magnetic insulators. Many explanations consider thermally excited magnons as the underling mechanism, for which direct evidence is missing so far. We present a systematic study of the SSE in Yttrium Iron Garnet (YIG) films of different thicknesses. From the thickness dependence of the measured inverse spin Hall effect we can unambiguously identify the SSE effect. Corresponding simulations on atomistic length scales allow us to deduce the propagation length of the thermally excited magnons, which could be used to manipulate domain walls.

  8. Nonreciprocal spin wave elementary excitation in dislocated dimerized Heisenberg chains.

    Science.gov (United States)

    Liu, Wanguo; Shen, Yang; Fang, Guisheng; Jin, Chongjun

    2016-05-18

    A mechanism for realizing nonreciprocal elementary excitation of spin wave (SW) is proposed. We study a reference model which describes a magnonic crystal (MC) formed by two Heisenberg chains with a lateral displacement (dislocation) and a longitudinal spacer, and derive a criterion to judge whether the elementary excitation spectra are reciprocal in this ferromagnetic lattice. An analytical method based on the spin precession equation is used to solve the elementary excitation spectra. The solution is related to a key factor, the spatio-temporal structure factor [Formula: see text], which can be directly calculated through the structural parameters. When it keeps invariant under the reversions of the external magnetic field [Formula: see text] and the dislocation [Formula: see text], or one of them, the spectra are reciprocal. Otherwise, the SW possesses nonreciprocal spectra with direction-dependent band edges and exhibits a directional magnetoresistance effect. This criterion can be regarded as a necessary and sufficient condition for the (non)reciprocity in the spin lattice. Besides, this novel lattice provides a prototype for spin diodes and spin logic gates.

  9. Spin Flips versus Spin Transport in Nonthermal Electrons Excited by Ultrashort Optical Pulses in Transition Metals

    Science.gov (United States)

    Shokeen, V.; Sanchez Piaia, M.; Bigot, J.-Y.; Müller, T.; Elliott, P.; Dewhurst, J. K.; Sharma, S.; Gross, E. K. U.

    2017-09-01

    A joint theoretical and experimental investigation is performed to understand the underlying physics of laser-induced demagnetization in Ni and Co films with varying thicknesses excited by 10 fs optical pulses. Experimentally, the dynamics of spins is studied by determining the time-dependent amplitude of the Voigt vector, retrieved from a full set of magnetic and nonmagnetic quantities performed on both sides of films, with absolute time reference. Theoretically, ab initio calculations are performed using time-dependent density functional theory. Overall, we demonstrate that spin-orbit induced spin flips are the most significant contributors with superdiffusive spin transport, which assumes only that the transport of majority spins without spin flips induced by scattering does not apply in Ni. In Co it plays a significant role during the first ˜20 fs only. Our study highlights the material dependent nature of the demagnetization during the process of thermalization of nonequilibrium spins.

  10. Excitations of incoherent spin-waves due to spin-transfer torque.

    Science.gov (United States)

    Lee, Kyung-Jin; Deac, Alina; Redon, Olivier; Nozières, Jean-Pierre; Dieny, Bernard

    2004-12-01

    The possibility of exciting microwave oscillations in a nanomagnet by a spin-polarized current, as predicted by Slonczewski and Berger, has recently been demonstrated. This observation opens important prospects of applications in radiofrequency components. However, some unresolved inconsistencies are found when interpreting the magnetization dynamics within the coherent spin-torque model. In some cases, the telegraph noise caused by spin-currents could not be quantitatively described by that model. This has led to controversy about the need for an effective magnetic temperature model. Here we interpret the experimental results of Kiselev et al. using micromagnetic simulations. We point out the key role played by incoherent spin-wave excitation due to spin-transfer torque. The incoherence is caused by spatial inhomogeneities in local fields generating distributions of local precession frequencies. We observe telegraph noise with gigahertz frequencies at zero temperature. This is a consequence of the chaotic dynamics and is associated with transitions between attraction wells in phase space.

  11. Crossover from spin waves to diffusive spin excitations in underdoped Ba(Fe1-xCox)2 As2

    Energy Technology Data Exchange (ETDEWEB)

    Tucker, G S; Fernandes, R M; Pratt, D K; Thaler, A; Ni, N; Marty, K; Christianson, A D; Lumsden, M D; Sales, B C; Sefat, A S; Bud' ko, S L; Canfield, P C; Kreyssig, A; Goldman, A I; McQueeney, R J

    2014-05-01

    Using inelastic neutron scattering, we show that the onset of superconductivity in underdoped Ba(Fe1-xCox)2As2 coincides with a crossover from well-defined spin waves to overdamped and diffusive spin excitations. This crossover occurs despite the presence of long-range stripe antiferromagnetic order for samples in a compositional range from x=0.04 to 0.055, and is a consequence of the shrinking spin-density wave gap and a corresponding increase in the particle-hole (Landau) damping. The latter effect is captured by a simple itinerant model relating Co doping to changes in the hot spots of the Fermi surface. We argue that the overdamped spin fluctuations provide a pairing mechanism for superconductivity in these materials.

  12. Spin Hall effect by surface roughness

    KAUST Repository

    Zhou, Lingjun

    2015-01-08

    The spin Hall and its inverse effects, driven by the spin orbit interaction, provide an interconversion mechanism between spin and charge currents. Since the spin Hall effect generates and manipulates spin current electrically, to achieve a large effect is becoming an important topic in both academia and industries. So far, materials with heavy elements carrying a strong spin orbit interaction, provide the only option. We propose here a new mechanism, using the surface roughness in ultrathin films, to enhance the spin Hall effect without heavy elements. Our analysis based on Cu and Al thin films suggests that surface roughness is capable of driving a spin Hall angle that is comparable to that in bulk Au. We also demonstrate that the spin Hall effect induced by surface roughness subscribes only to the side-jump contribution but not the skew scattering. The paradigm proposed in this paper provides the second, not if only, alternative to generate a sizable spin Hall effect.

  13. Collective Excitations in Spin-2 Bose-Einstein Condensates

    Institute of Scientific and Technical Information of China (English)

    HOU Jing-Min; TIAN Li-Jun

    2005-01-01

    The Green's functions and the correlation functions in spin-2 Bose-Einstein condensates at finite temperature are defined and the generalized Dyson-Beliaev equations are introduced. We discuss the spin conservation in z direction and decouple thre Green's functions and the generalized Dyson-Beliaev equations according to different spin conservations in z direction. The anomalous vertex functions are introduced and the self-energies are separated into the proper self-energies and the improper self-energies. The generalized Dyson-Beliaev equations are decoupled according to separation of the self-energies. We calculate the Green's functions step by step in the Bogoliubov approximation and discuss the collective excitations in spin-2 Bose-Einstein condensates in the polar, ferromagnetic, and cyclic cases,respectively.

  14. Generating Coherent Phonons and Spin Excitations with Ultrafast Light Pulses

    Science.gov (United States)

    Merlin, Roberto

    2006-03-01

    Recent work on the generation of coherent low-lying excitations by ultrafast laser pulses will be reviewed, emphasizing the microscopic mechanisms of light-matter interaction. The topics covered include long-lived phonons in ZnO [C. Aku-Leh, J. Zhao, R. Merlin, J. Men'endez and M. Cardona, Phys. Rev.B 71, 205211 (2005)], squeezed magnons [J. Zhao, A. V. Bragas, D. J. Lockwood and R. Merlin, Phys. Rev. Lett. 93, 107203 (2004)], spin- and charge-density fluctuations [J. M. Bao et al., Phys. Rev. Lett. 92, 236601 (2004)] and cyclotron resonance [J. K. Wahlstrand, D. M. Wang, P. Jacobs, J. M. Bao, R. Merlin, K. W. West and L. N. Pfeiffer, AIP Conference Proceedings 772 (2005), p. 1313] in GaAs quantum wells. In addition, unpublished results on surface -avoiding phonons in GaAs-AlAs superlattices [M. Trigo et al., unpublished] and magnons in ferromagnetic Ga1-xMnxAs [D. M. Wang et al., unpublished] will be discussed. It will also be shown that frequencies can be measured using pump-probe techniques with a precision comparable to that of Brillouin scattering. It is now widely accepted that stimulated Raman scattering (SRS) is (often but not always) the mechanism responsible for the coherent coupling. Results will be presented showing that SRS is described by two separate tensors, one of which accounts for the excitation-induced modulation of the susceptibility, and the other one for the dependence of the amplitude of the oscillation on the light intensity [T. E. Stevens, J. Kuhl and R. Merlin, Phys. Rev. B 65, 144304 (2002)]. These tensors have the same real component, associated with impulsive coherent generation, but different imaginary parts. If the imaginary term dominates, that is, for strongly absorbing substances, the mechanism for two-band processes becomes displacive in nature, as in the DECP (displacive excitation of coherent phonons) model. It will be argued that DECP is not a separate mechanism, but a particular case of SRS. In the final part of the talk, an

  15. The spin-flip extended single excitation configuration interaction method

    Science.gov (United States)

    Casanova, David; Head-Gordon, Martin

    2008-08-01

    An extension of the spin-flip single excitation configuration interaction (SF-CIS) method is introduced. The extension, abbreviated as SF-XCIS, includes all configurations in which no more than one virtual level of the high spin triplet reference becomes occupied and no more than one doubly occupied level becomes vacant. The number of such configurations is quadratic with molecule size, and the method is implemented in a direct algorithm whose cost scales in the same way with molecule size as CIS itself, thus permitting applications to large systems. Starting from a spin restricted triplet determinant, SF-XCIS yields spin-pure singlet, triplet, and quintet states, and treats both half-occupied reference orbitals in a fully balanced way to allow application to strongly correlated problems. Tests on bond dissociation in the HF molecule, the torsional potential of ethylene, and excited states of polyenes show encouraging improvements using SF-XCIS compared to SF-CIS and a previously suggested extension, the spin-complete CIS model.

  16. Nuclear Level Density at High Spin and Excitation Energy

    Institute of Scientific and Technical Information of China (English)

    A.N. Behkami; Z. Kargar

    2001-01-01

    The intensive studies of equilibrium processes in heavy-ion reaction have produced a need for information on nuclear level densities at high energies and spins. The Fermi gas level density is often used in investigation of heavy-ion reaction studies. Some papers have claimed that nuclear level densities might deviate substantially from the Fermi gas predications at excitations related to heavy-ion reactions. The formulae of calculation of the nuclear level density based on the theory of superconductivity are presented, special attention is paid to the dependence of the level density on the angular momentum. The spin-dependent nuclear level density is evaluated using the pairing interaction. The resulting level density for an average spin of 52h is evaluated for 155Er and compared with experimental data. Excellent agreement between experiment and theory is obtained.``

  17. Localized spin excitations in an antiferromagnetic spin system with D-M interaction

    Energy Technology Data Exchange (ETDEWEB)

    Evangeline Rebecca, T.; Latha, M. M., E-mail: lathaisaac@yahoo.com [Department of Physics, Women' s Christian College, Nagercoil 629 001 (India)

    2016-06-15

    The existence of localized spin excitations and spin deviations along the site in a one-dimensional antiferromagnet with Dzyaloshinski-Moriya (D-M) interaction has been studied using quasiclassical approximation. By introducing the Holstein-Primakoff bosonic representation of spin operators, the coherent state ansatz, and the time dependent variational principle, a discrete set of coupled nonlinear partial differential equations governing the dynamics is derived. Employing the multiple-scale method, one, two and three solitary wave solutions are constructed and depicted graphically.

  18. User-friendly software for modeling collective spin wave excitations

    Science.gov (United States)

    Hahn, Steven; Peterson, Peter; Fishman, Randy; Ehlers, Georg

    There exists a great need for user-friendly, integrated software that assists in the scientific analysis of collective spin wave excitations measured with inelastic neutron scattering. SpinWaveGenie is a C + + software library that simplifies the modeling of collective spin wave excitations, allowing scientists to analyze neutron scattering data with sophisticated models fast and efficiently. Furthermore, one can calculate the four-dimensional scattering function S(Q,E) to directly compare and fit calculations to experimental measurements. Its generality has been both enhanced and verified through successful modeling of a wide array of magnetic materials. Recently, we have spent considerable effort transforming SpinWaveGenie from an early prototype to a high quality free open source software package for the scientific community. S.E.H. acknowledges support by the Laboratory's Director's fund, ORNL. Work was sponsored by the Division of Scientific User Facilities, Office of Basic Energy Sciences, US Department of Energy, under Contract No. DE-AC05-00OR22725 with UT-Battelle, LLC.

  19. Spin excitations in hole-overdoped iron-based superconductors.

    Science.gov (United States)

    Horigane, K; Kihou, K; Fujita, K; Kajimoto, R; Ikeuchi, K; Ji, S; Akimitsu, J; Lee, C H

    2016-09-12

    Understanding the overall features of magnetic excitation is essential for clarifying the mechanism of Cooper pair formation in iron-based superconductors. In particular, clarifying the relationship between magnetism and superconductivity is a central challenge because magnetism may play a key role in their exotic superconductivity. BaFe2As2 is one of ideal systems for such investigation because its superconductivity can be induced in several ways, allowing a comparative examination. Here we report a study on the spin fluctuations of the hole-overdoped iron-based superconductors Ba1-xKxFe2As2 (x = 0.5 and 1.0; Tc = 36 K and 3.4 K, respectively) over the entire Brillouin zone using inelastic neutron scattering. We find that their spin spectra consist of spin wave and chimney-like dispersions. The chimney-like dispersion can be attributed to the itinerant character of magnetism. The band width of the spin wave-like dispersion is almost constant from the non-doped to optimum-doped region, which is followed by a large reduction in the overdoped region. This suggests that the superconductivity is suppressed by the reduction of magnetic exchange couplings, indicating a strong relationship between magnetism and superconductivity in iron-based superconductors.

  20. Spin excitations in hole-overdoped iron-based superconductors

    Science.gov (United States)

    Horigane, K.; Kihou, K.; Fujita, K.; Kajimoto, R.; Ikeuchi, K.; Ji, S.; Akimitsu, J.; Lee, C. H.

    2016-01-01

    Understanding the overall features of magnetic excitation is essential for clarifying the mechanism of Cooper pair formation in iron-based superconductors. In particular, clarifying the relationship between magnetism and superconductivity is a central challenge because magnetism may play a key role in their exotic superconductivity. BaFe2As2 is one of ideal systems for such investigation because its superconductivity can be induced in several ways, allowing a comparative examination. Here we report a study on the spin fluctuations of the hole-overdoped iron-based superconductors Ba1-xKxFe2As2 (x = 0.5 and 1.0; Tc = 36 K and 3.4 K, respectively) over the entire Brillouin zone using inelastic neutron scattering. We find that their spin spectra consist of spin wave and chimney-like dispersions. The chimney-like dispersion can be attributed to the itinerant character of magnetism. The band width of the spin wave-like dispersion is almost constant from the non-doped to optimum-doped region, which is followed by a large reduction in the overdoped region. This suggests that the superconductivity is suppressed by the reduction of magnetic exchange couplings, indicating a strong relationship between magnetism and superconductivity in iron-based superconductors. PMID:27615691

  1. Superconductivity and spin excitations in orbitally ordered FeSe

    Science.gov (United States)

    Kreisel, Andreas; Mukherjee, Shantanu; Hirschfeld, P. J.; Andersen, B. M.

    We provide a band-structure with low-energy properties consistent with recent photoemission and quantum oscillations measurements on the Fe-based superconductor FeSe, including a mean-field like orbital ordering in the dxz /dyz channel, and show that this model also accounts for the temperature dependence of the measured Knight shift and the spin-relaxation rate. An RPA calculation of the dynamical spin susceptibility yields spin excitations which are peaked at wave vector (π , 0) in the 1-Fe Brillouin zone, with a broad maximum at energies of order a few meV. Furthermore, the superconducting gap structure obtained from spin fluctuation theory exhibits nodes on the electron pockets, consistent with the 'V'-shaped density of states measured by tunneling spectroscopy on this material. The redistribution of spectral weight in the superconducting state creates a (π , 0) ''neutron resonance'' as seen in recent experiments. Comparing to various experimental results, we give predictions for further studies A.K. and B.M.A. acknowledge financial support from a Lundbeckfond fellowship (Grant No. A9318). P.J.H. was partially supported by the Department of Energy under Grant No. DE-FG02-05ER46236.

  2. Thermal Hall Effect of Spin Excitations in a Kagome Magnet.

    Science.gov (United States)

    Hirschberger, Max; Chisnell, Robin; Lee, Young S; Ong, N P

    2015-09-04

    At low temperatures, the thermal conductivity of spin excitations in a magnetic insulator can exceed that of phonons. However, because they are charge neutral, the spin waves are not expected to display a thermal Hall effect. However, in the kagome lattice, theory predicts that the Berry curvature leads to a thermal Hall conductivity κ(xy). Here we report observation of a large κ(xy) in the kagome magnet Cu(1-3, bdc) which orders magnetically at 1.8 K. The observed κ(xy) undergoes a remarkable sign reversal with changes in temperature or magnetic field, associated with sign alternation of the Chern flux between magnon bands. The close correlation between κ(xy) and κ(xx) firmly precludes a phonon origin for the thermal Hall effect.

  3. Resonant excitation of coupled skyrmions by spin-transfer torque

    Science.gov (United States)

    Dai, Y. Y.; Wang, H.; Yang, T.; Zhang, Z. D.

    2016-12-01

    Resonant excitations of coupled skyrmions in Co/Ru/Co nanodisks activated by spin-transfer torque (STT) have been studied by micromagnetic simulations. It is found that STT is an effective method to manipulate skyrmion dynamics. Unlike the dynamics driven by a microwave field, two skyrmions with opposite chiralities move synchronously in the same direction when they are driven by STT, which makes it easier to observe the dynamics of coupled skyrmions in experiments. Resonant excitations of coupled skyrmions can be controlled by changing the frequency or amplitude ratio of a dual-frequency alternating current (AC). In addition, the magnetostatic interaction between the two skyrmions plays an important role in the dynamics of coupled skyrmions.

  4. Low-spin excitations in {sup 146}Sm

    Energy Technology Data Exchange (ETDEWEB)

    Kueppersbusch, C.; Brentano, P. von; Endres, J.; Elvers, M.; Friessner, C.; Zell, K.O.; Zilges, A. [Universitaet zu Koeln, Institut fuer Kernphysik, Koeln (Germany); Pascu, S. [Universitaet zu Koeln, Institut fuer Kernphysik, Koeln (Germany); National Institute for Physics and Nuclear Engineering, Bucharest-Magurele (Romania); Bucurescu, D.; Deleanu, D.; Filipescu, D.; Ghita, D.G.; Glodariu, T.; Mihai, C.; Marginean, N.M.; Marginean, R.; Negret, A.; Sava, T.; Stroe, L.; Zamfir, N.V. [National Institute for Physics and Nuclear Engineering, Bucharest-Magurele (Romania); Cata-Danil, G. [National Institute for Physics and Nuclear Engineering, Bucharest-Magurele (Romania); University POLITEHNICA of Bucharest, Physics Department, Bucharest (Romania); Werner, V. [Yale University, Wright Nuclear Structure Laboratory, New Haven, Connecticut (United States)

    2012-01-15

    The low-spin excitations of the nucleus {sup 146}Sm which is just two neutrons and two protons away from the N = 82 shell and Z = 64 subshell closures have been investigated by means of the {sup 143}Nd({alpha},n) and {sup 144}Nd({alpha},2n) fusion-evaporation reactions. We established 47 hitherto unknown energy levels up to 4.7MeV and 75 new transitions. In addition, 7 spin assignments were possible from the {gamma}-{gamma} angular correlation analysis. The structure of the possible candidates for a 2{sup +} x 3{sup -} quadrupole-octupole multiplet are first discussed in terms of the harmonic vibrational model. A comparison of these states with the corresponding ones in the neighboring N=84 isotones is also presented. Finally, the structure of the {sup 146}Sm nucleus is interpreted in terms of the IBA-spdf model. It is shown that the model is able to reproduce the experimental relative transition strengths of the 2{sup +} x 3{sup -} quadrupole-octupole multiplet and also a series of collective properties such as the proposed double-octupole excitations. (orig.)

  5. Evidence for a spinon Fermi surface in a triangular-lattice quantum-spin-liquid candidate

    Science.gov (United States)

    Shen, Yao; Li, Yao-Dong; Wo, Hongliang; Li, Yuesheng; Shen, Shoudong; Pan, Bingying; Wang, Qisi; Walker, H. C.; Steffens, P.; Boehm, M.; Hao, Yiqing; Quintero-Castro, D. L.; Harriger, L. W.; Frontzek, M. D.; Hao, Lijie; Meng, Siqin; Zhang, Qingming; Chen, Gang; Zhao, Jun

    2016-12-01

    A quantum spin liquid is an exotic quantum state of matter in which spins are highly entangled and remain disordered down to zero temperature. Such a state of matter is potentially relevant to high-temperature superconductivity and quantum-information applications, and experimental identification of a quantum spin liquid state is of fundamental importance for our understanding of quantum matter. Theoretical studies have proposed various quantum-spin-liquid ground states, most of which are characterized by exotic spin excitations with fractional quantum numbers (termed ‘spinons’). Here we report neutron scattering measurements of the triangular-lattice antiferromagnet YbMgGaO4 that reveal broad spin excitations covering a wide region of the Brillouin zone. The observed diffusive spin excitation persists at the lowest measured energy and shows a clear upper excitation edge, consistent with the particle-hole excitation of a spinon Fermi surface. Our results therefore point to the existence of a quantum spin liquid state with a spinon Fermi surface in YbMgGaO4, which has a perfect spin-1/2 triangular lattice as in the original proposal of quantum spin liquids.

  6. Evidence for a spinon Fermi surface in a triangular-lattice quantum-spin-liquid candidate.

    Science.gov (United States)

    Shen, Yao; Li, Yao-Dong; Wo, Hongliang; Li, Yuesheng; Shen, Shoudong; Pan, Bingying; Wang, Qisi; Walker, H C; Steffens, P; Boehm, M; Hao, Yiqing; Quintero-Castro, D L; Harriger, L W; Frontzek, M D; Hao, Lijie; Meng, Siqin; Zhang, Qingming; Chen, Gang; Zhao, Jun

    2016-12-05

    A quantum spin liquid is an exotic quantum state of matter in which spins are highly entangled and remain disordered down to zero temperature. Such a state of matter is potentially relevant to high-temperature superconductivity and quantum-information applications, and experimental identification of a quantum spin liquid state is of fundamental importance for our understanding of quantum matter. Theoretical studies have proposed various quantum-spin-liquid ground states, most of which are characterized by exotic spin excitations with fractional quantum numbers (termed 'spinons'). Here we report neutron scattering measurements of the triangular-lattice antiferromagnet YbMgGaO4 that reveal broad spin excitations covering a wide region of the Brillouin zone. The observed diffusive spin excitation persists at the lowest measured energy and shows a clear upper excitation edge, consistent with the particle-hole excitation of a spinon Fermi surface. Our results therefore point to the existence of a quantum spin liquid state with a spinon Fermi surface in YbMgGaO4, which has a perfect spin-1/2 triangular lattice as in the original proposal of quantum spin liquids.

  7. Low-spin excitations in {sup 98}Ru

    Energy Technology Data Exchange (ETDEWEB)

    Radeck, Desiree; Albers, Michael; Bernards, Christian; Fransen, Christoph; Jolie, Jan; Muecher, Dennis [Institut fuer Kernphysik, Universitaet Koeln (Germany)

    2009-07-01

    In the context of collectivity in the A=100 mass region N=52 isotones were investigated in detail and phonon excitations - especially the mixed-symmetry (MS) states - were identified. In order to investigate how states with this MS character evolve with increasing valence neutron number N=54 isotones were studied. While in {sup 96}Mo the one-phonon MS state 2{sup +}{sub 1,ms} was identified, {sup 98}Ru shows a breakdown of vibrational structure above the two-phonon triplet and no candidate for the 2{sup +}{sub 1,ms} state was assigned. The recently investigated N=54 isotone {sup 100}Pd was explained well with an U{sub {pi}}{sub {nu}}(5) fit within the IBM-2. Furthermore, a candidate for the one-phonon MS2{sup +}{sub 1,ms} state was determined. To do further investigations on the N=54 isotone {sup 98}Ru - in particular regarding the breakdown of vibrational symmetry and the one-phonon MS excitation - an experiment was performed at the Cologne Tandem Accelerator using the HORUS spectrometer. The nuclei were populated by the reaction {sup 97}Mo({sup 3}He,2n){sup 98}Ru. By analysing the coincidence and {gamma}{gamma} angular correlation data the level scheme was extended and clarified by determining spins, multipole mixing ratios and branching ratios. The low-energy excitations of positive parity are discussed and compared to theoretical expectations. The results are compared with those for other N=54 isotones.

  8. Nanoparticle-textured surfaces from spin coating.

    Science.gov (United States)

    Weiss, R A; Zhai, X; Dobrynin, A V

    2008-05-20

    Rough surfaces composed of discrete but relatively uniform nanoparticles were prepared from a lightly sulfonated polystyrene ionomer by spin coating from tetrahydrofuran (THF) or a THF/methanol mixture onto a silica surface. The particle morphology is consistent with the spinodal decomposition of the film surface occurring during spin coating. The particles are well wetted to the silica, and if heated for a long time above the ionomer's glass-transition temperature, the particles flow and coalesce into a smooth, homogeneous film.

  9. Excitations and spin correlations near the interface of two three-dimensional Heisenberg antiferromagnets

    Energy Technology Data Exchange (ETDEWEB)

    Voropajeva, N., E-mail: niina.voropajeva@ut.ee [Institute of Physics, University of Tartu, Riia 142, 51014 Tartu (Estonia); Sherman, A., E-mail: alexei@fi.tartu.ee [Institute of Physics, University of Tartu, Riia 142, 51014 Tartu (Estonia)

    2012-09-03

    Magnetic excitations and spin correlations near the interface of two spin-1/2 Heisenberg antiferromagnets are considered using the spin-wave approximation. When the interaction between boundary spins differs essentially from exchange constants inside the antiferromagnets, quasi-two-dimensional spin waves appear in the near-boundary region. They eject bulk magnons from this region, thereby dividing the antiferromagnets into areas with different magnetic excitations. The decreased dimensionality of the near-boundary modes leads to amplified nearest-neighbor spin correlations in the interface area. -- Highlights: ► Excitations near the interface of two Heisenberg antiferromagnets are considered. ► Different quasi-two-dimensional spin waves may appear in the interface region. ► The interface modes eject bulk modes from the near-boundary region. ► The interface modes produce amplified spin correlations near the boundary.

  10. Persistent spin excitations in doped antiferromagnets revealed by resonant inelastic light scattering

    Science.gov (United States)

    Jia, C. J.; Nowadnick, E. A.; Wohlfeld, K.; Kung, Y. F.; Chen, C.-C.; Johnston, S.; Tohyama, T.; Moritz, B.; Devereaux, T. P.

    2014-02-01

    How coherent quasiparticles emerge by doping quantum antiferromagnets is a key question in correlated electron systems, whose resolution is needed to elucidate the phase diagram of copper oxides. Recent resonant inelastic X-ray scattering (RIXS) experiments in hole-doped cuprates have purported to measure high-energy collective spin excitations that persist well into the overdoped regime and bear a striking resemblance to those found in the parent compound, challenging the perception that spin excitations should weaken with doping and have a diminishing effect on superconductivity. Here we show that RIXS at the Cu L3-edge indeed provides access to the spin dynamical structure factor once one considers the full influence of light polarization. Further we demonstrate that high-energy spin excitations do not correlate with the doping dependence of Tc, while low-energy excitations depend sensitively on doping and show ferromagnetic correlations. This suggests that high-energy spin excitations are marginal to pairing in cuprate superconductors.

  11. Evaluation of excitation energy and spin from light charged particles multiplicities in heavy-ion collisions

    CERN Document Server

    Steckmeyer, J C; Grotowski, K; Pawowski, P; Aiello, S; Anzalone, A; Bini, M; Borderie, B; Bougault, R; Cardella, G; Casini, G; Cavallaro, S; Charvet, J L; Dayras, R; De Filippo, E; Durand, D; Femin, S; Frankland, J D; Galíchet, E; Geraci, M; Giustolisi, F; Guazzoni, P; Iacono-Manno, M; Lanzalone, G; Lanzan, G; Le Neindre, N; Lo Nigro, S; Lo Piano, F; Olmi, A; Pagano, A; Papa, M; Pârlog, M; Pasquali, G; Piantelli, S; Pirrone, S; Politi, G; Porto, F; Rivet, M F; Rizzo, F; Rosato, E; Roy, R; Sambataro, S; Sperduto, M L; Stefanini, A A; Sutera, C; Tamain, B; Vient, E; Volant, C; Wieleczko, J P; Zetta, L

    2005-01-01

    A simple procedure for evaluating the excitation energy and the spin transfer in heavy-ion dissipative collisions is proposed. It is based on a prediction of the GEMINI evaporation code : for a nucleus with a given excitation energy, the average number of emitted protons decreases with increasing spin, whereas the average number of alpha particles increases. Using that procedure for the reaction 107Ag+58Ni at 52 MeV/nucleon, the excitation energy and spin of quasi-projectiles have been evaluated. The results obtained in this way have been compared with the predictions of a model describing the primary dynamic stage of heavy-ion collisions.

  12. Search for excited spin-3/2 neutrinos at LHeC

    CERN Document Server

    Ozansoy, A; Çetinkaya, V

    2016-01-01

    We study the potential of the next $ep$ collider, namely LHeC, with two options $\\sqrt{s}=1.3$ TeV $\\sqrt{s}=1.98$ TeV, to search for excited spin-1/2 and spin-3/2 neutrinos. We calculate the single production cross section of excited spin-1/2 and spin-3/2 neutrinos according to their effective currents describing their interactions between gauge bosons and SM leptons. We choose the $\

  13. Comparison of calculation methods for the tunnel splitting at excited states of biaxial spin models

    Institute of Scientific and Technical Information of China (English)

    Cui Xiao-Bo; Chen Zhi-De

    2004-01-01

    We present the calculation and comparison of tunnel splitting at excited levels of biaxial spin models by various methods, including the generalized instanton method, the generalized path integral method for coherent spin states,the perturbation method, and the exact method by numerical diagonalization of the Hamiltonian. It is found that,for integer spin with spin number around 10, tunnel splitting predicted by the generalized path integral for coherent spin states is about 10-n times of the exact numerical result for the nth excited level, while the ratio of the results of the perturbation method and the exact numerical method diverges in the large spin limit. We thus conclude that the generalized instanton method is the best approximate way for calculating tunnel splitting in spin models.

  14. Local excitation of surface plasmon polaritons in random surface nanostructures

    DEFF Research Database (Denmark)

    Bozhevolnyi, S.I.; Volkov, V.S.; Boltasseva, Alexandra;

    2003-01-01

    We investigate local excitation of surface plasmon polaritons (SPPs) at a 55-nm-thick gold layer covered with randomly located scatterers (density similar to75 mum(-2)) by using an uncoated fiber tip of a near-field optical microscope as a radiation source and detecting the radiation scattered...

  15. Local excitation of surface plasmon polaritons in random surface nanostructures

    DEFF Research Database (Denmark)

    Bozhevolnyi, S.I.; Volkov, V.S.; Boltasseva, Alexandra

    2003-01-01

    We investigate local excitation of surface plasmon polaritons (SPPs) at a 55-nm-thick gold layer covered with randomly located scatterers (density similar to75 mum(-2)) by using an uncoated fiber tip of a near-field optical microscope as a radiation source and detecting the radiation scattered...

  16. Surface sensitivity of the spin Seebeck effect

    NARCIS (Netherlands)

    Aqeel, Aisha; Vera Marun, Ivan; van Wees, Bart; Palstra, Thomas

    2014-01-01

    We have investigated the influence of the interface quality on the spin Seebeck effect (SSE) of the bilayer system yttrium iron garnet (YIG)-platinum (Pt). The magnitude and shape of the SSE is strongly influenced by mechanical treatment of the YIG single crystal surface. We observe that the saturat

  17. Tracking excited-state charge and spin dynamics in iron coordination complexes

    DEFF Research Database (Denmark)

    Zhang, Wenkai; Alonso-Mori, Roberto; Bergmann, Uwe

    2014-01-01

    to spin state, can elucidate the spin crossover dynamics of [Fe(2,2'-bipyridine)(3)](2+) on photoinduced metal-to-ligand charge transfer excitation. We are able to track the charge and spin dynamics, and establish the critical role of intermediate spin states in the crossover mechanism. We anticipate......Crucial to many light-driven processes in transition metal complexes is the absorption and dissipation of energy by 3d electrons(1-4). But a detailed understanding of such non-equilibrium excited-state dynamics and their interplay with structural changes is challenging: a multitude of excited...... states and possible transitions result in phenomena too complex to unravel when faced with the indirect sensitivity of optical spectroscopy to spin dynamics(5) and the flux limitations of ultrafast X-ray sources(6,7). Such a situation exists for archetypal poly-pyridyl iron complexes, such as [Fe(2...

  18. Low-energy electrodynamics of novel spin excitations in the quantum spin ice Yb₂Ti₂O₇.

    Science.gov (United States)

    Pan, LiDong; Kim, Se Kwon; Ghosh, A; Morris, Christopher M; Ross, Kate A; Kermarrec, Edwin; Gaulin, Bruce D; Koohpayeh, S M; Tchernyshyov, Oleg; Armitage, N P

    2014-09-18

    In condensed matter systems, formation of long-range order (LRO) is often accompanied by new excitations. However, in many geometrically frustrated magnetic systems, conventional LRO is suppressed, while non-trivial spin correlations are still observed. A natural question to ask is then what is the nature of the excitations in this highly correlated state without broken symmetry? Frequently, applying a symmetry breaking field stabilizes excitations whose properties reflect certain aspects of the anomalous state without LRO. Here we report a THz spectroscopy study of novel excitations in quantum spin ice Yb2Ti2O7 under a directed magnetic field. At large positive fields, both right- and left-handed magnon and two-magnon-like excitations are observed. The g-factors of these excitations are dramatically enhanced in the low-field limit, showing a crossover of these states into features consistent with the quantum string-like excitations proposed to exist in quantum spin ice in small fields.

  19. Search for Excited Spin-3/2 Neutrinos at LHeC

    Directory of Open Access Journals (Sweden)

    A. Ozansoy

    2016-01-01

    Full Text Available We study the potential of the next ep collider, namely, LHeC, with two options s=1.3 TeV and s=1.98 TeV, to search for excited spin-1/2 and spin-3/2 neutrinos. We calculate the single production cross-section of excited spin-1/2 and spin-3/2 neutrinos according to their effective currents describing their interactions between gauge bosons and SM leptons. We choose the ν⋆→eW decay mode of excited neutrinos and W→jj decay mode of W-boson for the analysis. We put some kinematical cuts for the final state detectable particles and plot the invariant mass distributions for signal and the corresponding backgrounds. In order to obtain accessible limits for excited neutrino couplings, we show the f-f′ and ciV-ciA contour plots for excited spin-1/2 and excited spin-3/2 neutrinos, respectively.

  20. Spin state transitions upon visible and infrared excitation of ferric MbN{sub 3}

    Energy Technology Data Exchange (ETDEWEB)

    Helbing, Jan, E-mail: j.helbing@pci.uzh.ch [Physikalisch-Chemisches Institut, Universitaet Zuerich, Winterthurerstrasse 190, 8057 Zuerich (Switzerland)

    2012-03-02

    Highlights: Black-Right-Pointing-Pointer Visible heme and infrared ligand excitation change the spin state equilibrium of MbN{sub 3}. Black-Right-Pointing-Pointer The difference in ligand binding angle between high and low spin protein was measured. Black-Right-Pointing-Pointer Spin state changes take place on the time scale of vibrational relaxation of heme. Black-Right-Pointing-Pointer Heme vibrations may modulate the electronic and functional properties of the protein. - Abstract: When azide binds to ferric Myoglobin it forms either a low-spin or a high-spin complex, which give rise to two well-separated asymmetric stretch bands of the ligand. Both electronic excitation of the Q-band and vibrational excitation of N{sub 3}{sup -} in the mid-IR lead to a similar ultrafast population redistribution in favor of the high spin configuration, which is characterized by a 8 Degree-Sign reorientation of the ligand transition dipole moment. The more stable low spin complex subsequently re-emerges with a 18 ps time-constant. It is argued that the observed spin state changes are caused by the participation of low-lying electronic excitations in the cooling process of heme.

  1. Reversible quantum optical data storage based on resonant Raman optical field excited spin coherence.

    Science.gov (United States)

    Ham, Byoung S

    2008-09-01

    A method of reversible quantum optical data storage is presented using resonant Raman field excited spin coherence, where the spin coherence is stored in an inhomogeneously broadened spin ensemble. Unlike the photon echo method, in the present technique, a 2pi Raman optical rephasing pulse area is used and multimode (parallel) optical channels are available in which the multimode access gives a great benefit to quantum information processors such as quantum repeaters.

  2. Spin-dipole excitations studied with tensor polarised deuteron beams

    NARCIS (Netherlands)

    Wortche, H. J.; Julin, R; Demetriuo, P; Harissopulos, SV

    2008-01-01

    Taking advantage of the spin, isospin and J(pi) selectivity of cross sections and analysing powers of the tensor polarised C-12 (d(->), He-2) reaction, the J(pi) = 0(-), 1(-), 2(-) components of the spin-dipole resonance in B-12 have been investigated. The experiment was performed at the Big-Bite Sp

  3. Excitation and spin-transport of hot holes in ballistic hole magnetic microscopy

    NARCIS (Netherlands)

    Haq, E.; Banerjee, T.; Siekman, M.H.; Lodder, J.C.; Jansen, R.

    2006-01-01

    A hybrid structure of a ferromagnetic Co/Au/Ni81Fe19 trilayer on p-type silicon is used to probe the excitation of electron-hole pairs in a ferromagnet during inelastic decay of hot electrons and the subsequent spin-dependent transport of the excited holes into the valence band of the p-type Si coll

  4. Excitation Spectrum of Spin-1 Bosonic Atoms in Mott Insulating Phase

    Institute of Scientific and Technical Information of China (English)

    HOU Jing-Min; TIAN Li-Jun

    2006-01-01

    The effective action for spin-1 bosonic atom in an optical lattice is derived. The quasiparticle and quasihole dispersions are calculated for different cases by using a functional integral formalism. For all cases, the excitation spectra are analyzed. All the quasiparticle and quasihole excitations start with a gap.

  5. SPIN-ISOSPIN EXCITATIONS IN NUCLEI VIA (HE-3,T) REACTIONS AT 450 MEV

    NARCIS (Netherlands)

    FUJIWARA, M; AKIMUNE, H; DAITO, [No Value; EJIRI, H; FUJITA, Y; GREENFIELD, MB; HARAKEH, MN; HAZAMA, R; INOMATA, T; JANECKE, J; KUDOMI, N; KUME, K; NAKAYAMA, S; SHINMYO, K; TAMII, A; TANAKA, M; TOYOKAWA, H; YOSOI, M

    1994-01-01

    Spin-isospin excitations in nuclei havee been studied by means of the (He-3, t) reactions at 450 MeV. The Gamow-Teller (GT) resonances are found to be strongly excited. A fine structure of the giant Gamow Teller resonances in medium-heavy nuclei is observed with an energy resolution of 130 keV. The

  6. Effect of high-frequency excitation on natural frequencies of spinning discs

    DEFF Research Database (Denmark)

    Hansen, Morten Hartvig

    2000-01-01

    The effect of high-frequency, non-resonant parametric excitation on the low-frequency response of spinning discs is considered. The parametric excitation is obtained through a non-constant rotation speed, where the frequency of the pulsating overlay is much higher than the lowest natural frequenc...

  7. Hybrid excitations due to crystal field, spin-orbit coupling, and spin waves in LiFePO4

    Science.gov (United States)

    Yiu, Yuen; Le, Manh Duc; Toft-Peterson, Rasmus; Ehlers, Georg; McQueeney, Robert J.; Vaknin, David

    2017-03-01

    We report on the spin waves and crystal field excitations in single crystal LiFePO4 by inelastic neutron scattering over a wide range of temperatures, below and above the antiferromagnetic transition of this system. In particular, we find extra excitations below TN=50 K that are nearly dispersionless and are most intense around magnetic zone centers. We show that these excitations correspond to transitions between thermally occupied excited states of Fe2 + due to splitting of the S =2 levels that arise from the crystal field and spin-orbit interactions. These excitations are further amplified by the highly distorted nature of the oxygen octahedron surrounding the iron atoms. Above TN, magnetic fluctuations are observed up to at least 720 K, with an additional inelastic excitation around 4 meV, which we attribute to single-ion effects, as its intensity weakens slightly at 720 K compared to 100 K, which is consistent with the calculated cross sections using a single-ion model. Our theoretical analysis, using the MF-RPA model, provides both detailed spectra of the Fe d shell and estimates of the average ordered magnetic moment and TN. By applying the MF-RPA model to a number of existing spin-wave results from other Li M PO4 (M =Mn , Co, and Ni), we are able to obtain reasonable predictions for the moment sizes and transition temperatures.

  8. Spin excitations in systems with hopping electron transport and strong position disorder in a large magnetic field

    Science.gov (United States)

    Shumilin, A. V.

    2016-10-01

    We discuss the spin excitations in systems with hopping electron conduction and strong position disorder. We focus on the problem in a strong magnetic field when the spin Hamiltonian can be reduced to the effective single-particle Hamiltonian and treated with conventional numerical technics. It is shown that in a 3D system with Heisenberg exchange interaction the spin excitations have a delocalized part of the spectrum even in the limit of strong disorder, thus leading to the possibility of the coherent spin transport. The spin transport provided by the delocalized excitations can be described by a diffusion coefficient. Non-homogenous magnetic fields lead to the Anderson localization of spin excitations while anisotropy of the exchange interaction results in the Lifshitz localization of excitations. We discuss the possible effect of the additional exchange-driven spin diffusion on the organic spin-valve devices.

  9. Momentum and Doping Dependence of Spin Excitations in Electron-Doped Cuprate Superconductors

    Science.gov (United States)

    Jing, Pengfei; Zhao, Huaisong; Kuang, Lülin; Lan, Yu; Feng, Shiping

    2017-01-01

    Superconductivity in copper oxides emerges on doping holes or electrons into their Mott-insulating parent compounds. The spin excitations are thought to be the mediating glue for the pairing in superconductivity. Here the momentum and doping dependence of the dynamical spin response in the electron-doped cuprate superconductors is studied based on the kinetic-energy-driven superconducting mechanism. It is shown that the dispersion of the low-energy spin excitations changes strongly upon electron doping; however, the hour-glass-shaped dispersion of the low-energy spin excitations appeared in the hole-doped case is absent on the electron-doped side due to the electron-hole asymmetry. In particular, the commensurate resonance appears in the superconducting state with the resonance energy that correlates with the dome-shaped doping dependence of the superconducting gap. Moreover, the spectral weight and dispersion of the high-energy spin excitations in the superconducting state are comparable with those in the corresponding normal state, indicating that the high-energy spin excitations do not play an important part in the pair formation.

  10. Doping dependence of spin excitations and its correlations with high-temperature superconductivity in iron pnictides.

    Science.gov (United States)

    Wang, Meng; Zhang, Chenglin; Lu, Xingye; Tan, Guotai; Luo, Huiqian; Song, Yu; Wang, Miaoyin; Zhang, Xiaotian; Goremychkin, E A; Perring, T G; Maier, T A; Yin, Zhiping; Haule, Kristjan; Kotliar, Gabriel; Dai, Pengcheng

    2013-01-01

    High-temperature superconductivity in iron pnictides occurs when electrons and holes are doped into their antiferromagnetic parent compounds. Since spin excitations may be responsible for electron pairing and superconductivity, it is important to determine their electron/hole-doping evolution and connection with superconductivity. Here we use inelastic neutron scattering to show that while electron doping to the antiferromagnetic BaFe₂As₂ parent compound modifies the low-energy spin excitations and their correlation with superconductivity (100 meV), hole-doping suppresses the high-energy spin excitations and shifts the magnetic spectral weight to low-energies. In addition, our absolute spin susceptibility measurements for the optimally hole-doped iron pnictide reveal that the change in magnetic exchange energy below and above T(c) can account for the superconducting condensation energy. These results suggest that high-T(c) superconductivity in iron pnictides is associated with both the presence of high-energy spin excitations and a coupling between low-energy spin excitations and itinerant electrons.

  11. Spin dynamics of an individual Cr atom in a semiconductor quantum dot under optical excitation

    Energy Technology Data Exchange (ETDEWEB)

    Lafuente-Sampietro, A. [Université Grenoble Alpes, Institut Néel, F-38000 Grenoble (France); CNRS, Institut Néel, F-38000 Grenoble (France); Institute of Materials Science, University of Tsukuba, 305-8573 Tsukuba (Japan); Utsumi, H.; Kuroda, S. [Institute of Materials Science, University of Tsukuba, 305-8573 Tsukuba (Japan); Boukari, H.; Besombes, L., E-mail: lucien.besombes@grenoble.cnrs.fr [Université Grenoble Alpes, Institut Néel, F-38000 Grenoble (France); CNRS, Institut Néel, F-38000 Grenoble (France)

    2016-08-01

    We studied the spin dynamics of a Cr atom incorporated in a II-VI semiconductor quantum dot using photon correlation techniques. We used recently developed singly Cr-doped CdTe/ZnTe quantum dots to access the spin of an individual magnetic atom. Auto-correlation of the photons emitted by the quantum dot under continuous wave optical excitation reveals fluctuations of the localized spin with a timescale in the 10 ns range. Cross-correlation gives quantitative transfer time between Cr spin states. A calculation of the time dependence of the spin levels population in Cr-doped quantum dots shows that the observed spin dynamics is dominated by the exciton-Cr interaction. These measurements also provide a lower bound in the 20 ns range for the intrinsic Cr spin relaxation time.

  12. Simulating Quantum Spin Models using Rydberg-Excited Atomic Ensembles in Magnetic Microtrap Arrays

    CERN Document Server

    Whitlock, Shannon; Hannaford, Peter

    2016-01-01

    We propose a scheme to simulate lattice spin models based on strong and long-range interacting Rydberg atoms stored in a large-spacing array of magnetic microtraps. Each spin is encoded in a collective spin state involving a single $nP$ Rydberg atom excited from an ensemble of ground-state alkali atoms prepared via Rydberg blockade. After the excitation laser is switched off the Rydberg spin states on neighbouring lattice sites interact via general isotropic or anisotropic spin-spin interactions. To read out the collective spin states we propose a single Rydberg atom triggered avalanche scheme in which the presence of a single Rydberg atom conditionally transfers a large number of ground-state atoms in the trap to an untrapped state which can be readily detected by site-resolved absorption imaging. Such a quantum simulator should allow the study of quantum spin systems in almost arbitrary two-dimensional configurations. This paves the way towards engineering exotic spin models, such as spin models based on tr...

  13. On the spin excitation energy of the nucleon in the Skyrme model

    CERN Document Server

    Adam, C; Wereszczynski, A

    2016-01-01

    In the Skyrme model of nucleons and nuclei, the spin excitation energy of the nucleon is traditionally calculated by a fit of the rigid rotor quantization of spin/isospin of the fundamental Skyrmion (the hedgehog) to the masses of the nucleon and the Delta resonance. The resulting, quite large spin excitation energy of the nucleon of about $ 73\\, \\mbox{MeV}$ is, however, rather difficult to reconcile with the small binding energies of physical nuclei, among other problems. Here we argue that a more reliable value for the spin excitation energy of the nucleon, compatible with many physical constraints, is about $ 16\\, \\mbox{MeV}$. The fit of the rigid rotor to the Delta, on the other hand, is problematic in any case, because it implies the use of a nonrelativistic method for a highly relativistic system.

  14. Emergence of nontrivial magnetic excitations in a spin-liquid state of kagomé volborthite

    Science.gov (United States)

    Watanabe, Daiki; Sugii, Kaori; Shimozawa, Masaaki; Suzuki, Yoshitaka; Yajima, Takeshi; Ishikawa, Hajime; Hiroi, Zenji; Shibauchi, Takasada; Matsuda, Yuji; Yamashita, Minoru

    2016-08-01

    When quantum fluctuations destroy underlying long-range ordered states, novel quantum states emerge. Spin-liquid (SL) states of frustrated quantum antiferromagnets, in which highly correlated spins fluctuate down to very low temperatures, are prominent examples of such quantum states. SL states often exhibit exotic physical properties, but the precise nature of the elementary excitations behind such phenomena remains entirely elusive. Here, we use thermal Hall measurements that can capture the unexplored property of the elementary excitations in SL states, and report the observation of anomalous excitations that may unveil the unique features of the SL state. Our principal finding is a negative thermal Hall conductivity κxyκxy which the charge-neutral spin excitations in a gapless SL state of the 2D kagomé insulator volborthite Cu3V2O7(OH)2ṡṡ2H2O exhibit, in much the same way in which charged electrons show the conventional electric Hall effect. We find that κxyκxy is absent in the high-temperature paramagnetic state and develops upon entering the SL state in accordance with the growth of the short-range spin correlations, demonstrating that κxyκxy is a key signature of the elementary excitation formed in the SL state. These results suggest the emergence of nontrivial elementary excitations in the gapless SL state which feel the presence of fictitious magnetic flux, whose effective Lorentz force is found to be less than 1/100 of the force experienced by free electrons.

  15. Relativistic response and novel spin-charge plasmon at the Tl/Si(111) surface

    Science.gov (United States)

    Lafuente-Bartolome, Jon; Gurtubay, Idoia G.; Eiguren, Asier

    2017-07-01

    We present a comprehensive ab initio analysis of the spin-charge correlations at the Tl/Si(111) surface, where the spin-orbit interaction is so strong that a detailed treatment of the noncollinear electron spin appears decisive for the correct description of the response properties. The relativistic limit enforces a unified treatment of the spin and charge densities as a four-vector, and the response function acquires then a 4 ×4 tensor structure. Our all-electron implementation allows us to resolve the real-space structure of the possible collective modes, and demonstrates the emergence of a novel collective excitation combining transverse-spin and ordinary charge oscillations of a similar order of magnitude, whose spin character is strongly enhanced as we approach the q →0 momentum limit.

  16. Surface plasmon interference excited by tightly focused laser beams.

    Energy Technology Data Exchange (ETDEWEB)

    Bouhelier, A.; Ignatovich, F.; Bruyant, A.; Huang, C.; Colas des Francs, G.; Weeber, J.-C.; Dereux, A.; Wiederrecht, G. P.; Novotny, L.; Center for Nanoscale Materials; Univ de Bourgogne; Univ. of Rochester; Univ Technologique de Troyes

    2007-09-01

    We show that interfering surface plasmon polaritons can be excited with a focused laser beam at normal incidence to a plane metal film. No protrusions or holes are needed in this excitation scheme. Depending on the axial position of the focus, the intensity distribution on the metal surface is either dominated by interferences between counterpropagating plasmons or by a two-lobe pattern characteristic of localized surface plasmon excitation. Our experiments can be accurately explained by use of the angular spectrum representation and provide a simple means for locally exciting standing surface plasmon polaritons.

  17. Pumping of nuclear spins by optical excitation of spin-forbidden transitions in a quantum dot.

    Science.gov (United States)

    Chekhovich, E A; Makhonin, M N; Kavokin, K V; Krysa, A B; Skolnick, M S; Tartakovskii, A I

    2010-02-12

    We demonstrate that efficient optical pumping of nuclear spins in semiconductor quantum dots (QDs) can be achieved by resonant pumping of optically forbidden transitions. This process corresponds to one-to-one conversion of a photon absorbed by the dot into a polarized nuclear spin, and also has potential for initialization of hole spin in QDs. We find that by employing this spin-forbidden process, nuclear polarization of 65% can be achieved, markedly higher than from pumping the allowed transition, which saturates due to the low probability of electron-nuclear spin flip-flop.

  18. Spin torque on the surface of graphene in the presence of spin orbit splitting

    Directory of Open Access Journals (Sweden)

    Ji Chen

    2013-06-01

    Full Text Available We study theoretically the spin transfer torque of a ferromagnetic layer coupled to (deposited onto a graphene surface in the presence of the Rashba spin orbit coupling (RSOC. We show that the RSOC induces an effective magnetic field, which will result in the spin precession of conduction electrons. We derive correspondingly the generalized Landau-Lifshitz-Gilbert (LLG equation, which describes the precessional motion of local magnetization under the influence of the spin orbit effect. Our theoretical estimate indicates that the spin orbit spin torque may have significant effect on the magnetization dynamics of the ferromagnetic layer coupled to the graphene surface.

  19. Evolution of spin excitations in a gapped antiferromagnet from the quantum to the high-temperature limit

    DEFF Research Database (Denmark)

    Kenzelmann, M.; Cowley, R.A.; Buyers, W.J.L.

    2002-01-01

    is in agreement with quantum Monte Carlo calculations for the spin-1 chain. xi is also consistent with the single mode approximation, suggesting that the excitations are short-lived single particle excitations. Below T=12 K where three-dimensional spin correlations are important, xi is shorter than predicted......We have mapped from the quantum to the classical limit the spin excitation spectrum of the antiferromagnetic spin-1 Heisenberg chain system CsNiCl3 in its paramagnetic phase from T=5 to 200 K. Neutron scattering shows that the excitations are resonant and dispersive up to at least T=70 Ksimilar...

  20. Magnetic correlation, excitation and slow dynamics in concentrated spin-glass alloys

    Indian Academy of Sciences (India)

    Kiyoichiro Motoya

    2004-07-01

    Three kinds of neutron scattering experiments have been performed to clarify the role of magnetic clusters on the various properties of re-entrant spin-glasses. The presence of two kinds of spin-wave excitations, the limitations of magnetic phase diagrams and the mechanism of slow dynamics have been discussed based on the results of in-elastic scattering, diffuse scattering and time-resolved small-angle scattering experiments, respectively.

  1. Ground Band and Excited Band of Spin-1 BEC in Cigar Shaped Laser Trap

    Institute of Scientific and Technical Information of China (English)

    PANG Wei; LI Zhi-Bing; BAO Cheng-Guang

    2007-01-01

    The wavefunctions that conserve the total spin are constructed for the fully condensed states and the states with one particle excited. A set of equations are deduced for the spatial longitudinal wavefunctions and the chemical potentials. These equations are solved numerically for 23Na and 87Rb condensates. The deformed trap shows significant effects on the spectrum. This implies that the spin effect of the spinor BEC are more easily detected in an optical trap of larger aspect ratio.

  2. Strong Linear Dichroism in Spin-Polarized Photoemission from Spin-Orbit-Coupled Surface States

    Science.gov (United States)

    Bentmann, H.; Maaß, H.; Krasovskii, E. E.; Peixoto, T. R. F.; Seibel, C.; Leandersson, M.; Balasubramanian, T.; Reinert, F.

    2017-09-01

    A comprehensive understanding of spin-polarized photoemission is crucial for accessing the electronic structure of spin-orbit coupled materials. Yet, the impact of the final state in the photoemission process on the photoelectron spin has been difficult to assess in these systems. We present experiments for the spin-orbit split states in a Bi-Ag surface alloy showing that the alteration of the final state with energy may cause a complete reversal of the photoelectron spin polarization. We explain the effect on the basis of ab initio one-step photoemission theory and describe how it originates from linear dichroism in the angular distribution of photoelectrons. Our analysis shows that the modulated photoelectron spin polarization reflects the intrinsic spin density of the surface state being sampled differently depending on the final state, and it indicates linear dichroism as a natural probe of spin-orbit coupling at surfaces.

  3. Spin induced gigahertz polarization oscillations in vertical-cavity surface-emitting laser devices

    Science.gov (United States)

    Li, M. Y.; Jaehme, H.; Soldat, H.; Gerhardt, N. C.; Hofmann, M. R.; Ackemann, T.

    2011-03-01

    Spin-controlled vertical-cavity surface-emitting lasers (VCSELs) have been intensively studied in recent years because of the low threshold feasibility and the nonlinearity above threshold, which make spin-VCSELs very promising for spintronic devices. Here we investigate the circular polarization dynamics of VCSELs on a picosecond time scale after pulsed optical spin injection at room temperature. A hybrid excitation technique combining continuous-wave (cw) unpolarized electrical excitation slightly above threshold and pulsed polarized optical excitation is applied. The experimental results demonstrate ultrafast circular polarization oscillations with a frequency of about 11 GHz. The oscillations last inside the first undulation of the intensity relaxation oscillations. Via theoretical calculations based on a rate equation model we analyze these oscillations as well as the underlying physical mechanisms.

  4. Spin Waves Excitations of Co/Pt Multilayers

    Directory of Open Access Journals (Sweden)

    W. Zhou

    2012-01-01

    Full Text Available The present work investigated interlayer couplings of [Co(20 Å/Pt(30 Å]5, [Co(4 Å/Pt(7 Å]30, and [Co(4 Å/Pt(9 Å]30 multilayers with strong perpendicular magnetic anisotropy (PMA. Brillouin light scattering measurements were utilized to obtain spin waves of these samples with in-plane external magnetic fields. Interlayer couplings were found to be very sensitive to Pt thickness change from 7 Å to 9 Å, which implies that Pt atoms were more difficult to be polarized to provide interlayer coupling between Co layers than in the perpendicular external magnetic field situation. When Pt layer is 30 Å, the observed single spin wave can confirm the disappearance of interlayer coupling even when Co layer thickness is 20 Å.

  5. Lifetime measurement of excited low-spin states via the $(p,p^{\\prime}\\gamma$) reaction

    CERN Document Server

    Hennig, A; Mineva, M N; Petkov, P; Pickstone, S G; Spieker, M; Zilges, A

    2015-01-01

    In this article a method for lifetime measurements in the sub-picosecond regime via the Doppler-shift attenuation method (DSAM) following the inelastic proton scattering reaction is presented. In a pioneering experiment we extracted the lifetimes of 30 excited low-spin states of $^{96}$Ru, taking advantage of the coincident detection of scattered protons and de-exciting $\\gamma$-rays as well as the large number of particle and $\\gamma$-ray detectors provided by the SONIC@HORUS setup at the University of Cologne. The large amount of new experimental data shows that this technique is suited for the measurement of lifetimes of excited low-spin states, especially for isotopes with a low isotopic abundance, where $(n,n^{\\prime}\\gamma$) or - in case of investigating dipole excitations - ($\\gamma,\\gamma^{\\prime}$) experiments are not feasible due to the lack of sufficient isotopically enriched target material.

  6. Statistical mechanics of magnetic excitations from spin waves to stripes and checkerboards

    CERN Document Server

    Rastelli, Enrico

    2013-01-01

    The aim of this advanced textbook is to provide the reader with a comprehensive explanation of the ground state configurations, the spin wave excitations and the equilibrium properties of spin lattices described by the Ising-Heisenberg Hamiltonians in the presence of short (exchange) and long range (dipole) interactions.The arguments are presented in such detail so as to enable advanced undergraduate and graduate students to cross the threshold of active research in magnetism by using both analytic calculations and Monte Carlo simulations.Recent results about unorthodox spin configurations suc

  7. Storage of Multiple Coherent Microwave Excitations in an Electron Spin Ensemble

    DEFF Research Database (Denmark)

    Wu, Hua; George, Richard E.; Wesenberg, Janus H.;

    2010-01-01

    stored and retrieved. Here we employ holographic techniques to realize a coherent memory using a pulsed magnetic field gradient and demonstrate the storage and retrieval of up to 100 weak 10 GHz coherent excitations in collective states of an electron spin ensemble. We further show that such collective......Strong coupling between a microwave photon and electron spins, which could enable a long-lived quantum memory element for superconducting qubits, is possible using a large ensemble of spins. This represents an inefficient use of resources unless multiple photons, or qubits, can be orthogonally...

  8. Excited-State Spin Manipulation and Intrinsic Nuclear Spin Memory using Single Nitrogen-Vacancy Centers in Diamond

    Science.gov (United States)

    Fuchs, Gregory

    2011-03-01

    Nitrogen vacancy (NV) center spins in diamond have emerged as a promising solid-state system for quantum information processing and precision metrology at room temperature. Understanding and developing the built-in resources of this defect center for quantum logic and memory is critical to achieving these goals. In the first case, we use nanosecond duration microwave manipulation to study the electronic spin of single NV centers in their orbital excited-state (ES). We demonstrate ES Rabi oscillations and use multi-pulse resonant control to differentiate between phonon-induced dephasing, orbital relaxation, and coherent electron-nuclear interactions. A second resource, the nuclear spin of the intrinsic nitrogen atom, may be an ideal candidate for a quantum memory due to both the long coherence of nuclear spins and their deterministic presence. We investigate coherent swaps between the NV center electronic spin state and the nuclear spin state of nitrogen using Landau-Zener transitions performed outside the asymptotic regime. The swap gates are generated using lithographically fabricated waveguides that form a high-bandwidth, two-axis vector magnet on the diamond substrate. These experiments provide tools for coherently manipulating and storing quantum information in a scalable solid-state system at room temperature. We gratefully acknowledge support from AFOSR, ARO, and DARPA.

  9. Collective spin excitation in finite size array of patterned magnonic crystals

    Energy Technology Data Exchange (ETDEWEB)

    Piao, H.-G. [College of Science, China Three Gorges University, Yichang 443002 (China); Shim, J.-H. [Department of Physics, Chungbuk National University, Cheongju 361-763 (Korea, Republic of); Pan, L. [College of Science, China Three Gorges University, Yichang 443002 (China); Yu, S.-C. [Department of Physics, Chungbuk National University, Cheongju 361-763 (Korea, Republic of); Kim, D.-H., E-mail: donghyun@chungbuk.ac.kr [Department of Physics, Chungbuk National University, Cheongju 361-763 (Korea, Republic of)

    2016-04-01

    We explore further details of the collectively excited spin wave mode in finite arrays of elliptically shaped ferromagnetic nanoelements as two-dimensional magnonic crystals by means of micromagnetic simulations. Under a pulsed magnetic driving field, collective spin wave modes were intensively investigated with variation of nanoelement dimensions and interelement separation as structural parameters of the magnonic crystal as well as changing the applied bias magnetic field. Via observing and analyzing the dynamic behavior of collective spin wave modes, we have found that the dynamic behavior strongly depends on the bias magnetic field with a quasi-linear dependency. The quasi-linear dependency of spin wave frequency transition can be achieved to a high sensitivity of the pT/Hz level. By modulating the magnonic crystal lattice structures and the bias magnetic field, the spin wave dynamic behavior is tunable which might be a promising property for a future magnonic crystal application and multifunctional sensors.

  10. Influence of interlayer coupling on the spin-torque-driven excitations in a spin-torque oscillator

    Science.gov (United States)

    Romera, M.; Monteblanco, E.; Garcia-Sanchez, F.; Delaët, B.; Buda-Prejbeanu, L. D.; Ebels, U.

    2017-03-01

    The influence of dynamic interlayer interactions on the spin-torque-driven and damped excitations are illustrated for a three layer macrospin model system that corresponds to a standard spin-torque oscillator. The free layer and a synthetic antiferromagnetic (SyF) pinned layer of the spin-torque oscillator are in-plane magnetized. In order to understand experimental results, numerical simulations have been performed considering three types of interlayer interactions: exchange interaction between the two magnetic layers of the SyF, mutual spin torque between the top layer of the SyF and the free layer and dipolar interaction between all three magnetic layers. It will be shown that the dynamic dipolar coupling plays a predominant role. First, it leads to a hybridization of the free layer and the SyF linear modes and through this gives rise to a strong field dependence of the critical current. In particular, there is a field range of enhanced damping in which much higher current is required to drive the modes into steady state. This results in a gap in the excitation spectrum. Second, the dynamic dipolar interaction is also responsible for the non-linear interaction between the current driven steady state mode and the damped modes of the system. Here one can distinguish: (i) a resonant interaction that leads to a kink in the frequency-field and frequency-current dispersions accompanied by a small hysteresis and a reduction of the linewidth of the steady state mode and (ii) a non-resonant interaction that leads to a strong frequency redshift of the damped mode. The results underline the strong impact of interlayer coupling on the excitation spectra of spin-torque oscillators and illustrate in a simple three mode model system how in the non-linear regime the steady state and damped modes influence each other.

  11. Surface sensitivity of the spin Seebeck effect

    Energy Technology Data Exchange (ETDEWEB)

    Aqeel, A.; Vera-Marun, I. J.; Wees, B. J. van; Palstra, T. T. M., E-mail: t.t.m.palstra@rug.nl [Zernike Institute for Advanced Materials, University of Groningen, Nijenborgh 4, 9747 AG Groningen (Netherlands)

    2014-10-21

    We have investigated the influence of the interface quality on the spin Seebeck effect (SSE) of the bilayer system yttrium iron garnet (YIG)–platinum (Pt). The magnitude and shape of the SSE is strongly influenced by mechanical treatment of the YIG single crystal surface. We observe that the saturation magnetic field (H{sub sat}{sup SSE}) for the SSE signal increases from 55.3 mT to 72.8 mT with mechanical treatment. The change in the magnitude of H{sub sat}{sup SSE} can be attributed to the presence of a perpendicular magnetic anisotropy due to the treatment induced surface strain or shape anisotropy in the Pt/YIG system. Our results show that the SSE is a powerful tool to investigate magnetic anisotropy at the interface.

  12. Coupling a Surface Acoustic Wave to an Electron Spin in Diamond via a Dark State

    Directory of Open Access Journals (Sweden)

    D. Andrew Golter

    2016-12-01

    Full Text Available The emerging field of quantum acoustics explores interactions between acoustic waves and artificial atoms and their applications in quantum information processing. In this experimental study, we demonstrate the coupling between a surface acoustic wave (SAW and an electron spin in diamond by taking advantage of the strong strain coupling of the excited states of a nitrogen vacancy center while avoiding the short lifetime of these states. The SAW-spin coupling takes place through a Λ-type three-level system where two ground spin states couple to a common excited state through a phonon-assisted as well as a direct dipole optical transition. Both coherent population trapping and optically driven spin transitions have been realized. The coherent population trapping demonstrates the coupling between a SAW and an electron spin coherence through a dark state. The optically driven spin transitions, which resemble the sideband transitions in a trapped-ion system, can enable the quantum control of both spin and mechanical degrees of freedom and potentially a trapped-ion-like solid-state system for applications in quantum computing. These results establish an experimental platform for spin-based quantum acoustics, bridging the gap between spintronics and quantum acoustics.

  13. Emission of correlated electron pairs from Au(111) and Cu(111) surfaces under low-energy electron impact: Contribution of surface states, d-states and spin effects

    Energy Technology Data Exchange (ETDEWEB)

    Samarin, S., E-mail: samar@physics.uwa.edu.au [Centre for Atomic, Molecular and Surface Physics, University of Western Australia, Perth, WA 6009 (Australia); Research Institute of Physics, St. Petersburg University, St. Petersburg (Russian Federation); Artamonov, O.M. [Research Institute of Physics, St. Petersburg University, St. Petersburg (Russian Federation); Guagliardo, P. [Centre for Microscopy, Characterisation and Analysis, UWA, Perth (Australia); Pravica, L. [Centre for Atomic, Molecular and Surface Physics, University of Western Australia, Perth, WA 6009 (Australia); Baraban, A. [Research Institute of Physics, St. Petersburg University, St. Petersburg (Russian Federation); Schumann, F.O. [Max-Planck-Institut für Mikrostrukturphysik, Weinberg 2, D-06120 Halle (Germany); Williams, J.F. [Centre for Atomic, Molecular and Surface Physics, University of Western Australia, Perth, WA 6009 (Australia)

    2015-01-15

    Highlights: • Spin-polarized two-electron spectroscopy (e,2e) was applied for studying surface states on Cu(111) and Au(111). • Relative (to d-states) contribution of surface states in the (e,2e) spectrum decreases exponentially when primary electron energy increases from 14 to 30 eV. • Spin asymmetry is readily observed in the spectra of Au(111) whereas in the spectra of Cu(111) the spin effect is negligible. - Abstract: The emission of correlated electron pairs excited from surfaces of Au(111) and Cu(111) by low-energy electrons is measured and analyzed. Energy and momentum conservation allows identification of electron pairs involving excitation of electrons from Shockley surface states and from valence d-states. The relative contributions of surface and d-states to the measured spectra of correlated electron pairs is shown to depend on the primary electron energy and is larger from surface states at relatively small primary energies. The use of a spin-polarized incident electron beam highlights the spin effects in producing an electron pair. Measurements show that spin effects are larger for the pair excitation from the valence d-states than for pairs excited from the surface states.

  14. Spin Chirality and Hall-Like Transport Phenomena of Spin Excitations

    Science.gov (United States)

    Han, Jung Hoon; Lee, Hyunyong

    2017-01-01

    Experimental and theoretical aspects of Hall-type transport of spins in magnetic insulators are reviewed. A general formalism for linear response theory of thermal Hall transport in the spin model is developed, which is general enough to be applicable to both the magnon and the paramagnetic, spin-liquid regimes. The expression of the energy current operator in the spin language is shown to be closely related to the spin chirality operator. Recent experiments on magnon-mediated thermal Hall transport in the two-dimensional kagome, and three-dimensional pyrochlore ferromagnetic insulators are reviewed in light of the multi-band magnon theory of Hall transport, and compared to the more mysterious thermal Hall transport found in the putative quantum spin ice material. As realizations of spin-chirality driven magnon transport in the real space, we review the general theory of emergent gauge fields governing the magnon dynamics in the textured magnet, and discuss its application to the magnon-Skyrmion scattering problem. Topological magnon Hall effect driven by the Skyrmion texture is discussed.

  15. Bounds on the electromagnetic interactions of excited spin-3/2 leptons

    CERN Document Server

    Walsh, R

    1999-01-01

    We discuss possible deviations from QED produced by a virtual excited spin-3/2 lepton in the reaction $e^+e^- \\longrightarrow 2\\gamma$. Data recorded by the OPAL Collaboration at a c.m. energy $\\sqrt{s} = 183 GeV$ are used to establish bounds on the nonstandard-lepton mass and coupling strengths.

  16. Excited state nonlinear integral equations for an integrable anisotropic spin-1 chain

    Energy Technology Data Exchange (ETDEWEB)

    Suzuki, J [Department of Physics, Faculty of Science, Shizuoka University, Ohya 836, Shizuoka (Japan)

    2004-12-17

    We propose a set of nonlinear integral equations to describe the excited states of an integrable the spin-1 chain with anisotropy. The scaling dimensions, evaluated numerically in previous studies, are recovered analytically by using the equations. This result may be relevant to the study of the supersymmetric sine-Gordon model.

  17. Ultrafast spin-transfer torque driven by femtosecond pulsed-laser excitation

    Science.gov (United States)

    Koopmans, Bert

    A hot topic in the field of ultrafast laser-induced manipulation of the magnetic state is that of the role and exploitation of laser-induced spin currents. Intense debate has been triggered by claims that such a spin-transfer, e.g. in the form of super-diffusive spin currents over tens of nanometers, might be a main contributor to the demagnetization process in ferromagnetic thin films after femtosecond laser excitation. In this presentation the underlying concepts will be introduced and recent developments reviewed. Particularly we demonstrate the possibility to apply a laser-induced spin transfer torque on a free magnetic layer, using a non-collinear multilayer configuration consisting of a free in-plane layer on top of a perpendicularly magnetized injection layer, as separated by a nonmagnetic spacer. Interestingly, this approach allows for a quantitative measurement of the amount of spin transfer. Moreover, it might provide access to novel device architectures in which the magnetic state is controlled by fs laser pulses. Careful analysis of the resulting precession of the free layer allows us to quantify the applied torque, and distinguish between driving mechanisms based on laser-induced transfer of hot electrons versus a spin Seebeck effect due to the large thermal gradients. Further engineering of the layered structures in order to gain fundamental understanding and optimize efficiencies will be reported. A simple model that treats local non-equilibrium magnetization dynamics to spin transport effects via a spin-dependent chemical potential will be introduced.

  18. Magnetic excitations and anomalous spin-wave broadening in multiferroic FeV2O4

    Energy Technology Data Exchange (ETDEWEB)

    Zhang, Qiang [Ames Laboratory; Ramazanoglu, Mehmet [Ames Laboratory; Chi, Songxue [Oak Ridge National Laboratory; Liu, Yong [Ames Laboratory; Lograsso, Thomas A. [Ames Laboratory; Vaknin, David [Ames Laboratory

    2014-06-01

    We report on the different roles of two orbital-active Fe2+ at the A site and V3+ at the B site in the magnetic excitations and on the anomalous spin-wave broadening in FeV2O4. FeV2O4 exhibits three structural transitions and successive paramagnetic (PM)–collinear ferrimagnetic (CFI)–noncollinear ferrimagnetic (NCFI)/ferroelectric transitions. The high-temperature tetragonal/PM–orthorhombic/CFI transition is accompanied by the appearance of a large energy gap in the magnetic excitations due to strong spin-orbit-coupling-induced anisotropy at the Fe2+ site. While there is no measurable increase in the energy gap from the orbital ordering of V3+ at the orthorhombic/CFI–tetragonal/NCFI transition, anomalous spin-wave broadening is observed in the orthorhombic/CFI state due to V3+ spin fluctuations at the B site. The spin-wave broadening is also observed at the zone boundary without softening in the NCFI/ferroelectric phase, which is discussed in terms of magnon-phonon coupling. Our study also indicates that the Fe2+ spins without the frustration at the A site may not play an important role in inducing ferroelectricity in the tetragonal/NCFI phase of FeV2O4.

  19. Enhanced spin Seebeck effect signal due to spin-momentum locked topological surface states

    Science.gov (United States)

    Jiang, Zilong; Chang, Cui-Zu; Masir, Massoud Ramezani; Tang, Chi; Xu, Yadong; Moodera, Jagadeesh S.; MacDonald, Allan H.; Shi, Jing

    2016-05-01

    Spin-momentum locking in protected surface states enables efficient electrical detection of magnon decay at a magnetic-insulator/topological-insulator heterojunction. Here we demonstrate this property using the spin Seebeck effect (SSE), that is, measuring the transverse thermoelectric response to a temperature gradient across a thin film of yttrium iron garnet, an insulating ferrimagnet, and forming a heterojunction with (BixSb1-x)2Te3, a topological insulator. The non-equilibrium magnon population established at the interface can decay in part by interactions of magnons with electrons near the Fermi energy of the topological insulator. When this decay channel is made active by tuning (BixSb1-x)2Te3 into a bulk insulator, a large electromotive force emerges in the direction perpendicular to the in-plane magnetization of yttrium iron garnet. The enhanced, tunable SSE which occurs when the Fermi level lies in the bulk gap offers unique advantages over the usual SSE in metals and therefore opens up exciting possibilities in spintronics.

  20. Spin-wave excitations and magnetism of sputtered Fe/Au multilayers

    Indian Academy of Sciences (India)

    M LASSRI; H SALHI; R MOUBAH; H LASSRI

    2016-08-01

    The spin-wave excitations and the magnetism of Fe/Au multilayers with different Fe thicknesses (tFe) grown by RF sputtering were investigated. The temperature dependence of spontaneous magnetization is well described by a T$_{3/2}$ law in all multilayers in the temperature range of 5–300 K. Spin-wave theory has been used to explain the temperature dependence of the spontaneous magnetization and the approximate values for the exchangeinteractions for various $t_{\\rm Fe}$ were obtained. The spin-wave constant $B$ was found to increase linearly with the inverse in the Fe thickness ($1/t_{\\rm Fe}$). Using the ferromagnetic resonance technique, the change of the anisotropy field $H_K$ as a function of $1/t_{\\rm Fe}$ was deduced. The spatial distributions of the discrete spin-wave modes were calculated. All theextracted results were in agreement with those determined experimentally and found in the literature.

  1. Excitation of bond-alternating spin-1/2 Heisenberg chains by tunnelling electrons.

    Science.gov (United States)

    Gauyacq, J-P; Lorente, N

    2014-10-01

    Inelastic electron tunneling spectra (IETS) are evaluated for spin-1/2 Heisenberg chains showing different phases of their spin ordering. The spin ordering is controlled by the value of the two different Heisenberg couplings on the two sides of each of the chain's atoms (bond-alternating chains). The perfect anti-ferromagnetic phase, i.e. a unique exchange coupling, marks a topological quantum phase transition (TQPT) of the bond-alternating chain. Our calculations show that the TQPT is recognizable in the excited states of the chain and hence that IETS is in principle capable of discriminating the phases. We show that perfectly symmetric chains, such as closed rings mimicking infinite chains, yield the same spectra on both sides of the TQPT and IETS cannot reveal the nature of the spin phase. However, for finite size open chains, both sides of the TQPT are associated with different IETS spectra, especially on the edge atoms, thus outlining the transition.

  2. Spin transport in undoped InGaAs/AlGaAs multiple quantum well studied via spin photocurrent excited by circularly polarized light.

    Science.gov (United States)

    Zhu, Laipan; Liu, Yu; Huang, Wei; Qin, Xudong; Li, Yuan; Wu, Qing; Chen, Yonghai

    2016-12-01

    The spin diffusion and drift at different excitation wavelengths and different temperatures have been studied in undoped InGaAs/AlGaAs multiple quantum well (MQW). The spin polarization was created by optical spin orientation using circularly polarized light, and the reciprocal spin Hall effect was employed to measure the spin polarization current. We measured the ratio of the spin diffusion coefficient to the mobility of spin-polarized carriers. From the wavelength dependence of the ratio, we found that the spin diffusion and drift of holes became as important as electrons in this undoped MQW, and the ratio for light holes was much smaller than that for heavy holes at room temperature. From the temperature dependence of the ratio, the correction factors for the common Einstein relationship for spin-polarized electrons and heavy holes were firstly obtained to be 93 and 286, respectively.

  3. Skew Scattering from Correlated Systems: Impurities and Collective Excitations in the Spin Hall Effect

    Science.gov (United States)

    Ziman, Timothy; Gu, Bo; Maekawa, Sadamichi

    2017-01-01

    The spin Hall effect is affected by the Coulomb interaction as well as spin-spin correlations in metals. Here we examine the enhancement in the effect caused by resonant skew scattering induced by electron correlations. For single-impurity scattering, local Coulomb correlations may significantly change the observed spin Hall angle. There may be additional effects because of the special atomic environment close to a surface — extra degeneracies compared to the bulk, enhanced correlations that move the relative d- or f-levels, and interference effects coming from the lower local dimension. Our results may explain the very large spin Hall angle observed in CuBi alloys. We discuss the impact on the spin Hall effect from cooperative effects, firstly in an itinerant ferromagnet where there is an anomaly near the Curie temperature originating from high-order spin fluctuations. The second case considered is a metallic spin glass, where exchange via slowly fluctuating magnetic moments may lead to the precession of an injected spin current. This decreases the net spin-charge conversion from skew scattering at temperatures below a value three or four times the freezing temperature.

  4. Renormalization of Optical Excitations in Molecules near a Metal Surface

    DEFF Research Database (Denmark)

    García Lastra, Juan Maria; Thygesen, Kristian Sommer

    2011-01-01

    The lowest electronic excitations of benzene and a set of donor-acceptor molecular complexes are calculated for the gas phase and on the Al(111) surface using the many-body Bethe-Salpeter equation. The energy of the charge-transfer excitations obtained for the gas phase complexes are found to be ...

  5. Continuous excitations of the triangular-lattice quantum spin liquid YbMgGaO4

    Science.gov (United States)

    Paddison, Joseph A. M.; Daum, Marcus; Dun, Zhiling; Ehlers, Georg; Liu, Yaohua; Stone, Matthew B.; Zhou, Haidong; Mourigal, Martin

    2016-12-01

    A quantum spin liquid (QSL) is an exotic state of matter in which electrons’ spins are quantum entangled over long distances, but do not show magnetic order in the zero-temperature limit. The observation of QSL states is a central aim of experimental physics, because they host collective excitations that transcend our knowledge of quantum matter; however, examples in real materials are scarce. Here, we report neutron-scattering experiments on YbMgGaO4, a QSL candidate in which Yb3+ ions with effective spin-1/2 occupy a triangular lattice. Our measurements reveal a continuum of magnetic excitations--the essential experimental hallmark of a QSL--at very low temperature (0.06 K). The origin of this peculiar excitation spectrum is a crucial question, because isotropic nearest-neighbour interactions do not yield a QSL ground state on the triangular lattice. Using measurements in the field-polarized state, we identify antiferromagnetic next-nearest-neighbour interactions, spin-space anisotropies, and chemical disorder between the magnetic layers as key ingredients in YbMgGaO4.

  6. Quantum Interference of Dual-Channel Excited Magnons in Spin-1 Bose—Einstein Condensates Atomic Chain

    Science.gov (United States)

    Zhao, Xu; Zhao, Xing-Dong; Zhou, Lu; Jing, Hui; Zhang, Wei-Ping

    2013-07-01

    We investigate the quantum interference of spin wave excitations of a spin-1 atomic Bose condensate confined in an optical lattice. Single-channel and dual-channel interactions are employed in our system, and their induced excitations are compared. Also we consider the interplay of magneto-optical excitations, which leads to a constructive or destructive effect for the creation of magnons based on background excitations. The population distributions of excited magnons can be well controlled by steering the long-range dipole-dipole interactions. Such a scheme can be used to demonstrate conventional quantum-optical phenomena like dynamical Casimir effect at finite temperatures.

  7. Quantum Interference of Dual-Channel Excited Magnons in Spin-1 Bose-Einstein Condensates Atomic Chain

    Institute of Scientific and Technical Information of China (English)

    ZHAO Xu; ZHAO Xing-Dong; ZHOU Lu; JING Hui; ZHANG Wei-Ping

    2013-01-01

    We investigate the quantum interference of spin wave excitations of a spin-1 atomic Bose condensate confined in an optical lattice.Single-channel and dual-channel interactions are employed in our system,and their induced excitations are compared.Also we consider the interplay of magneto-optical excitations,which leads to a constructive or destructive effect for the creation of magnons based on background excitations.The population distributions of excited magnons can be well controlled by steering the long-range dipole-dipole interactions.Such a scheme can be used to demonstrate conventional quantum-optical phenomena like dynamical Casimir effect at finite temperatures.

  8. Efficiency of local surface plasmon polariton excitation on ridges

    DEFF Research Database (Denmark)

    Radko, Ilya; Bozhevolnyi, Sergey I.; Boltasseva, Alexandra

    2008-01-01

    We investigate experimentally and numerically the efficiency of surface plasmon polariton excitation by a focused laser beam using gold ridges. The dependence of the efficiency on geometrical parameters of ridges and wavelength dependence are examined. The experimental measurements accomplished...

  9. Spin excitations and the electronic specific heat of URu2Si2

    DEFF Research Database (Denmark)

    Mason, T.E.; Buyers, W.J.L.

    1991-01-01

    and conduction electrons yields m*/m(b) almost-equal-to 7.7 for T T(N) which is sufficient to account for the difference between band-structure calculations and the measured electronic specific heat. In addition, inclusion of the temperature dependence of the spin...... excitations as T(N) is approached from below reproduces, qualitatively, the peak observed in the specific heat at T(N). The peak arises from a gap in the spin, not charge spectrum below T(N)....

  10. Non-thermal optical excitation of terahertz-spin precession in a magneto-optical insulator

    Energy Technology Data Exchange (ETDEWEB)

    Parchenko, Sergii; Maziewski, Andrzej; Stupakiewicz, Andrzej, E-mail: and@uwb.edu.pl [Laboratory of Magnetism, Faculty of Physics, University of Bialystok, 15-245 Bialystok (Poland); Satoh, Takuya [Department of Physics, Kyushu University, 819-0395 Fukuoka (Japan); Yoshimine, Isao [Institute of Industrial Science, The University of Tokyo, 153-8505 Tokyo (Japan); Stobiecki, Feliks [Institute of Molecular Physics Polish Academy of Sciences, 60-179 Poznan (Poland)

    2016-01-18

    We demonstrate non-thermal ultrafast laser excitation of spin precession with THz frequency in Gd-Bi-substituted iron garnet via the inverse Faraday effect. The modulation of THz precession by about 60 GHz below the compensation temperature of magnetic moment was observed. The THz frequency precession was caused by the exchange resonance between the Gd and Fe sublattices; we attributed the low-frequency modulation to dielectric resonance mode with a magnetic contribution. We demonstrate the possibility of polarization-sensitive control of spin precession under THz generation by laser pulses, helping to develop high-speed magneto-optical devices.

  11. Anomalous spin excitation spectrum of the Heisenberg model in a magnetic field.

    Science.gov (United States)

    Syljuåsen, Olav F; Lee, Patrick A

    2002-05-20

    Making the assumption that high-energy fermions exist in the two dimensional spin- 1/2 Heisenberg antiferromagnet, we present predictions based on the pi-flux ansatz for the dynamic structure factor when the antiferromagnet is subject to a uniform magnetic field. The main result is the presence of gapped excitations in a momentum region near (pi,pi) with energy lower than that at (pi,pi). This is qualitatively different from spin-wave theory predictions and may be tested by experiments or by quantum Monte Carlo.

  12. Spinon excitations in the spin-1 XXZ chain and hidden supersymmetry

    CERN Document Server

    Matsui, Chihiro

    2016-01-01

    We study spinon excitations of the integrable spin-1 (Fateev-Zamolodchikov; FZ) chain and their relation to the hidden supersymmetry. Using the notion of the supercharges earlier introduced to the spin chains, which change the system length by one, we found that they nontrivially act on one of two kinds of the degrees of freedom for the FZ chain. Their actions were obtained to be the same as those of the supercharges defined on the supersymmetric sine-Gordon model, the low-energy effective field theory of the FZ chain. Moreover, we construct the eigenstates which are invariant under the supersymmetric Hamiltonian given as the anti-commutator of the supercharges.

  13. Excitation Spectrum of Spin-1 Bosonic Atoms in an Optical Lattice with High Filling Factors

    Institute of Scientific and Technical Information of China (English)

    HOU Jing-Min

    2007-01-01

    The Green's function and the higher-order correlation functions of spin-1 cold atoms in an optical lattice are defined.Because we consider the problem of spin-1 Bose condensed atoms in an optical lattice with high filling factors,I.e.,the number density of Bose condensed atoms no is large,the fluctuation of them can be neglected and we take mean-field approximation for the higher-order terms.The excitation spectra for both the polar case and the ferromagnetic case are obtained and analyzed.

  14. Perturbed soliton spin excitations by EM-field in ferromagnetic medium

    CERN Document Server

    Daniel, M

    2003-01-01

    We study nonlinear spin excitations in the form of perturbed solitons in a one dimensional inhomogeneous bilinear anisotropic Heisenberg ferromagnet and an anisotropic homogeneous biquadratic ferromagnet in the classical continuum limit when acted upon by an electromagnetic(EM)-field. Using a reductive perturbation method, we deduce the associated Landau-Lifshtiz equations coupled with Maxwell's equations to perturbed nonlinear Schroedinger equations. A perturbation analysis carried out in both cases shows that the EM-field excites the magnetization of the medium in the form of solitons with small fluctuations.

  15. Stable oscillation in spin torque oscillator excited by a small in-plane magnetic field

    Energy Technology Data Exchange (ETDEWEB)

    Taniguchi, Tomohiro; Tsunegi, Sumito; Kubota, Hitoshi [National Institute of Advanced Industrial Science and Technology (AIST), Spintronics Research Center, Tsukuba 305-8568 (Japan); Ito, Takahiro; Utsumi, Yasuhiro [Faculty of Engineering, Mie University, Tsu, Mie 514-8507 (Japan)

    2015-08-07

    Theoretical conditions to excite self-oscillation in a spin torque oscillator consisting of a perpendicularly magnetized free layer and an in-plane magnetized pinned layer are investigated by analytically solving the Landau-Lifshitz-Gilbert equation. The analytical relation between the current and oscillation frequency is derived. It is found that a large amplitude oscillation can be excited by applying a small field pointing to the direction anti-parallel to the magnetization of the pinned layer. The validity of the analytical results is confirmed by comparing with numerical simulation, showing good agreement especially in a low current region.

  16. Spin clusters and low-energy excitations in rare earth kagome systems

    Science.gov (United States)

    Hoch, M. J. R.

    2017-01-01

    The rare earth kagome systems R3Ga5SiO14 (R = Nd or Pr), which are weakly frustrated antiferromagnets, do not exhibit long-range order at temperatures down to 40 mK as revealed by neutron scattering. The neutron experiments provide evidence for the emergence at low temperatures of correlated spins in nanoscale cluster regions with magnetic field-dependent correlation lengths. A variety of techniques have been used to determine the magnetic and thermal properties of these systems. In particular, high-field electron spin resonance (ESR), nuclear magnetic resonance (NMR) and muon spin resonance (μSR) experiments have established that dynamic correlation of spins remains significant at temperatures well above 1 K. ESR provides evidence for spin wave excitations in spin clusters and the spectra have been interpreted using a Heisenberg model approach. While Nd3+ (J = 9/2) is a Kramers ion Pr3+ (J = 4) is not. This difference leads to contrasts in the magnetic properties of the two systems. This review surveys the information that has been obtained on the properties of these kagome materials over the past decade.

  17. Thermal phase transition in artificial spin ice systems induces the formation and migration of monopole-like magnetic excitations

    Science.gov (United States)

    León, Alejandro

    2016-11-01

    Artificial spin ice systems exhibit monopole-like magnetic excitations. We develop here a theoretical study of the thermal phase transition of an artificial spin ice system, and we elucidate the role of the monopole excitations in the transition temperature. The dynamics of the spin ice is described by an efficient model based on cellular automata, which considers both thermal effects and dipolar interactions. We have established the critical temperature of the phase transition as function of the magnetic moment and the energy barrier of reversion. In addition, we predict that thermal gradients in the system induce the motion of elementary excitations, which could permit to manipulate monopole-like states.

  18. Thermal phase transition in artificial spin ice systems induces the formation and migration of monopole-like magnetic excitations

    Energy Technology Data Exchange (ETDEWEB)

    León, Alejandro

    2016-11-01

    Artificial spin ice systems exhibit monopole-like magnetic excitations. We develop here a theoretical study of the thermal phase transition of an artificial spin ice system, and we elucidate the role of the monopole excitations in the transition temperature. The dynamics of the spin ice is described by an efficient model based on cellular automata, which considers both thermal effects and dipolar interactions. We have established the critical temperature of the phase transition as function of the magnetic moment and the energy barrier of reversion. In addition, we predict that thermal gradients in the system induce the motion of elementary excitations, which could permit to manipulate monopole-like states.

  19. Equation-of-motion coupled cluster method for the description of the high spin excited states

    Science.gov (United States)

    Musiał, Monika; Lupa, Łukasz; Kucharski, Stanisław A.

    2016-04-01

    The equation-of-motion (EOM) coupled cluster (CC) approach in the version applicable for the excitation energy (EE) calculations has been formulated for high spin components. The EE-EOM-CC scheme based on the restricted Hartree-Fock reference and standard amplitude equations as used in the Davidson diagonalization procedure yields the singlet states. The triplet and higher spin components require separate amplitude equations. In the case of quintets, the relevant equations are much simpler and easier to solve. Out of 26 diagrammatic terms contributing to the R1 and R2 singlet equations in the case of quintets, only R2 operator survives with 5 diagrammatic terms present. In addition all terms engaging three body elements of the similarity transformed Hamiltonian disappear. This indicates a substantial simplification of the theory. The implemented method has been applied to the pilot study of the excited states of the C2 molecule and quintet states of C and Si atoms.

  20. Damped spin excitations in a doped cuprate superconductor with orbital hybridization

    DEFF Research Database (Denmark)

    Ivashko, O.; Shaik, N. E.; Lu, X.

    2017-01-01

    A resonant inelastic x-ray scattering study of overdamped spin excitations in slightly underdoped La2-xSrxCuO4 (LSCO) with x = 0.12 and 0.145 is presented. Three high-symmetry directions have been investigated: (1) the antinodal (0,0) -> (½,0), (2) the nodal (0,0) -> (¼, ¼), and (3) the zone-boun...

  1. Structural analysis of [Fe(ptz) sub 6)](BF sub 4) sub 2 under photo-excitation. Condensation of photo-excited high-spin ions

    CERN Document Server

    Moritomo, Y; Sakata, M; Kato, K; Kuriki, A; Nakamoto, A; Kojima, N

    2002-01-01

    We have performed in situ synchrotron-radiation X-ray powder structural analysis in a spin-crossover complex ([Fe(ptz) sub 6](BF sub 4) sub 2 : ptz=propyltetrazole) under a photo-excitation with a continuous-wave (CW) green (532 nm) laser at 91 K. The Fe sup 2 sup + ions in the Fe(ptz) sub 6 molecules take the low-spin (LS: S=0) state at the ground state, and are photo-excited selectively into the high-spin (HS: S=2) state. When the excitation power P exceeds the critical value, we observed a novel secondary phase which can be ascribed to the condensation of the photo-excited HS ions. (author)

  2. Edge physics of the quantum spin Hall insulator from a quantum dot excited by optical absorption.

    Science.gov (United States)

    Vasseur, Romain; Moore, Joel E

    2014-04-11

    The gapless edge modes of the quantum spin Hall insulator form a helical liquid in which the direction of motion along the edge is determined by the spin orientation of the electrons. In order to probe the Luttinger liquid physics of these edge states and their interaction with a magnetic (Kondo) impurity, we consider a setup where the helical liquid is tunnel coupled to a semiconductor quantum dot that is excited by optical absorption, thereby inducing an effective quantum quench of the tunneling. At low energy, the absorption spectrum is dominated by a power-law singularity. The corresponding exponent is directly related to the interaction strength (Luttinger parameter) and can be computed exactly using boundary conformal field theory thanks to the unique nature of the quantum spin Hall edge.

  3. Fully Suspended, Five-Axis, Three-Magnetic-Bearing Dynamic Spin Rig With Forced Excitation

    Science.gov (United States)

    Morrison, Carlos R.; Provenza, Andrew; Kurkov, Anatole; Montague, Gerald; Duffy, Kirsten; Mehmed, Oral; Johnson, Dexter; Jansen, Ralph

    2004-01-01

    The Five-Axis, Three-Magnetic-Bearing Dynamic Spin Rig, a significant advancement in the Dynamic Spin Rig (DSR), is used to perform vibration tests of turbomachinery blades and components under rotating and nonrotating conditions in a vacuum. The rig has as its critical components three magnetic bearings: two heteropolar radial active magnetic bearings and a magnetic thrust bearing. The bearing configuration allows full vertical rotor magnetic suspension along with a feed-forward control feature, which will enable the excitation of various natural blade modes in bladed disk test articles. The theoretical, mechanical, electrical, and electronic aspects of the rig are discussed. Also presented are the forced-excitation results of a fully levitated, rotating and nonrotating, unbladed rotor and a fully levitated, rotating and nonrotating, bladed rotor in which a pair of blades was arranged 180 degrees apart from each other. These tests include the bounce mode excitation of the rotor in which the rotor was excited at the blade natural frequency of 144 Hz. The rotor natural mode frequency of 355 Hz was discerned from the plot of acceleration versus frequency. For nonrotating blades, a blade-tip excitation amplitude of approximately 100 g/A was achieved at the first-bending critical (approximately 144 Hz) and at the first-torsional and second-bending blade modes. A blade-tip displacement of 70 mils was achieved at the first-bending critical by exciting the blades at a forced-excitation phase angle of 908 relative to the vertical plane containing the blades while simultaneously rotating the shaft at 3000 rpm.

  4. Ultrafast Optical Excitation of a Persistent Surface-State Population in the Topological Insulator Bi2Se3

    Energy Technology Data Exchange (ETDEWEB)

    Sobota, Jonathan

    2012-03-14

    Using femtosecond time- and angle-resolved photoemission spectroscopy, we investigated the nonequilibrium dynamics of the topological insulator Bi{sub 2}Se{sub 3}. We studied p-type Bi{sub 2}Se{sub 3}, in which the metallic Dirac surface state and bulk conduction bands are unoccupied. Optical excitation leads to a meta-stable population at the bulk conduction band edge, which feeds a nonequilibrium population of the surface state persisting for >10 ps. This unusually long-lived population of a metallic Dirac surface state with spin texture may present a channel in which to drive transient spin-polarized currents.

  5. Direct mapping of spin and orbital entangled wave functions under interband spin-orbit coupling of giant Rashba spin-split surface states

    Science.gov (United States)

    Noguchi, Ryo; Kuroda, Kenta; Yaji, K.; Kobayashi, K.; Sakano, M.; Harasawa, A.; Kondo, Takeshi; Komori, F.; Shin, S.

    2017-01-01

    We use spin- and angle-resolved photoemission spectroscopy (SARPES) combined with a polarization-variable laser and investigate the spin-orbit coupling effect under interband hybridization of Rashba spin-split states for the surface alloys Bi/Ag(111) and Bi/Cu(111). In addition to the conventional band mapping of photoemission for Rashba spin splitting, the different orbital and spin parts of the surface wave function are directly imaged into energy-momentum space. It is unambiguously revealed that the interband spin-orbit coupling modifies the spin and orbital character of the Rashba surface states leading to the enriched spin-orbital entanglement and the pronounced momentum dependence of the spin polarization. The hybridization thus strongly deviates the spin and orbital characters from the standard Rashba model. The complex spin texture under interband spin-orbit hybridization proposed by first-principles calculation is experimentally unraveled by SARPES with a combination of p - and s -polarized light.

  6. A Magnetic Suspension and Excitation System for Spin Vibration Testing of Turbomachinery Blades

    Science.gov (United States)

    Johnson, Dexter; Brown, Gerald V.; Mehmed, Oral

    1998-01-01

    The Dynamic Spin Rig (DSR) is used to perform vibration tests of turbomachinery blades and components under spinning conditions in a vacuum. A heteropolar radial active magnetic bearing was integrated into the DSR to provide non-contact magnetic suspension and mechanical excitation of the rotor to induce turbomachinery blade vibrations. The magnetic bearing replaces one of the two existing conventional radial ball bearings. Prior operation of the DSR used two voice-coil type linear electromagnetic shakers which provided axial excitation of the rotor. The new magnetic suspension and excitation system has provided enhanced testing capabilities. Tests were performed at high rotational speeds for longer duration and higher vibration amplitudes. Some characteristics of the system include magnetic bearing stiffness values up to 60,000 lb./in., closed loop control bandwidth around 500 Hz, and multi-directional radial excitation of the rotor. This paper reports on the implementation and operation of this system and presents some test results using this system.

  7. Investigation of surface magnetic noise by shallow spins in diamond.

    Science.gov (United States)

    Rosskopf, T; Dussaux, A; Ohashi, K; Loretz, M; Schirhagl, R; Watanabe, H; Shikata, S; Itoh, K M; Degen, C L

    2014-04-11

    We present measurements of spin relaxation times (T1, T1ρ, T2) on very shallow (≲5  nm) nitrogen-vacancy centers in high-purity diamond single crystals. We find a reduction of spin relaxation times up to 30 times compared to bulk values, indicating the presence of ubiquitous magnetic impurities associated with the surface. Our measurements yield a density of 0.01-0.1μB/nm2 and a characteristic correlation time of 0.28(3) ns of surface states, with little variation between samples and chemical surface terminations. A low temperature measurement further confirms that fluctuations are thermally activated. The data support the atomistic picture where impurities are associated with the top carbon layers, and not with terminating surface atoms or adsorbate molecules. The low spin density implies that the presence of a single surface impurity is sufficient to cause spin relaxation of a shallow nitrogen-vacancy center.

  8. Selective excitation of adsorbate vibrations on dissipative surfaces

    OpenAIRE

    2008-01-01

    The selective infrared (IR) excitation of molecular vibrations is a powerful tool to control the photoreactivity prior to electronic excitation in the ultraviolet / visible (UV/Vis) light regime ("vibrationally mediated chemistry"). For adsorbates on surfaces it has been theoretically predicted that IR preexcitation will lead to higher UV/Vis photodesorption yields and larger cross sections for other photoreactions. In a recent experiment, IR-mediated desorption of molecular hydrogen from a S...

  9. Transient Loschmidt Echo and Orthogonality Catastrophe in highly excited Quantum Ising Spin Chains

    Science.gov (United States)

    Schiro, Marco; Lupo, Carla

    We study the response to sudden local perturbations of highly excited Quantum Ising Spin Chains. The key quantity encoding this response is the overlap between time-dependent wave functions, which we write as a transient Loschmidt echo. We compute the Echo perturbatively in the case of a weak local quench and study its asymptotics at long times, which contains crucial information about the structure of the highly excited non-equilibrium environment induced by the quench. Our results reveal that the Echo decays exponentially, rather than power law as in the low-energy Orthogonality Catastrophe, a further example of quench-induced decoherence. The emerging decoherence scale is set by the strenght of the local potential and the bulk excitation energy. In addition, the transient evolution features aging behavior at the Ising quantum critical point.

  10. Spin contamination-free N-electron wave functions in the excitation-based configuration interaction treatment.

    Science.gov (United States)

    Alcoba, Diego R; Torre, Alicia; Lain, Luis; Massaccesi, Gustavo E; Oña, Ofelia B; Capuzzi, Pablo

    2016-07-07

    This work deals with the spin contamination in N-electron wave functions provided by the excitation-based configuration interaction methods. We propose a procedure to ensure a suitable selection of excited N-electron Slater determinants with respect to a given reference determinant, required in these schemes. The procedure guarantees the construction of N-electron wave functions which are eigenfunctions of the spin-squared operator Sˆ(2), avoiding any spin contamination. Our treatment is based on the evaluation of the excitation level of the determinants by means of the expectation value of an excitation operator formulated in terms of spin-free replacement operators. We report numerical determinations of energies and 〈Sˆ(2)〉 expectation values, arising from our proposal as well as from traditional configuration interaction methods, in selected open-shell systems, in order to compare the behavior of these procedures and their computational costs.

  11. Spin-state transition in LaCoO3: direct neutron spectroscopic evidence of excited magnetic states.

    Science.gov (United States)

    Podlesnyak, A; Streule, S; Mesot, J; Medarde, M; Pomjakushina, E; Conder, K; Tanaka, A; Haverkort, M W; Khomskii, D I

    2006-12-15

    A gradual spin-state transition occurs in LaCoO3 around T approximately 80-120 K, whose detailed nature remains controversial. We studied this transition by means of inelastic neutron scattering and found that with increasing temperature an excitation at approximately 0.6 meV appears, whose intensity increases with temperature, following the bulk magnetization. Within a model including crystal-field interaction and spin-orbit coupling, we interpret this excitation as originating from a transition between thermally excited states located about 120 K above the ground state. We further discuss the nature of the magnetic excited state in terms of intermediate-spin (t(2g)(5)e(g)(1), S=1) versus high-spin (t(2g)(4)e(g)(2), S=2) states. Since the g factor obtained from the field dependence of the inelastic neutron scattering is g approximately 3, the second interpretation is definitely favored.

  12. Dynamic magnetization switching and spin wave excitations by voltage-induced torque

    Science.gov (United States)

    Shiota, Yoichi

    2013-03-01

    The effect of electric fields on ultrathin ferromagnetic metal layer is one of the promising approaches for manipulating the spin direction with low-energy consumption, localization, and coherent behavior. Several experimental approaches to realize it have been investigated using ferromagnetic semiconductors, magnetostriction together with piezo-electric materials, multiferroic materials, and ultrathin ferromagnetic layer. In this talk, we will present a dynamic control of spins by voltage-induced torque. We used the magnetic tunnel junctions with ultrathin ferromagnetic layer, which shows voltage-induced perpendicular magnetic anisotropy change. By applying the voltage to the junction, the magnetic easy-axis in the ultrathin ferromagnetic layer changes from in-plane to out-of-plane, which causes a precession of the spins. This precession resulted in a two-way toggle switching by determining an appropriate pulse length. On the other hand, an application of rf-voltage causes an excitation of a uniform spin-wave. Since the precession of spin associates with an oscillation in the resistance of the junction, the applied rf-signal is rectified and produces a dc-voltage. From the spectrum of the dc-voltage as a function of frequency, we could estimate the voltage-induced torque. This research was supported by CREST-JST, G-COE program, and JSPS for the fellowship. Collaborators include T. Nozaki, S. Miwa, F. Bonell, N. Mizuochi, T. Shinjo, and Y. Suzuki.

  13. Long wavelength perturbations and excitations at surfaces

    Science.gov (United States)

    Kohn, W.

    Andre Blandin and I had been close frieds since the early 1960's and his death, following many very difficult years, is a deep personal loss for me. We had several strong common scientific interests which I enjoyed very much discussing with him : the effects of impurities on nuclear magnetic resonance; the electronic structure of alloys; and the theory of surfaces. I am pleased, as a tribute to the memory of a uniquely humane person and of a brilliant scientist to offer this paper. André Blandin et moi-même avons été des amis très proches depuis le début des années 1960 et sa mort, consécutive à de nombreuses années très difficiles, est pour moi une profonde perte personnelle. Nous avions de nombreux et forts intérets communs de nature scientifique, que je prenais plaisir à discuter avec lui : effets d'impuretés sur la résonance magnétique nucléaire, structure électronique des alliages et théorie des surfaces. Je suis heureux de contribuer par cet article à la mémoire d'un être aux qualités humaines uniques et d'un scientifique brillant.

  14. Unconventional Fermi surface spin patterns in the (Bi/Pb/Sb)/Ag(111) surface alloy

    Energy Technology Data Exchange (ETDEWEB)

    Meier, Fabian; Dil, Hugo [Physik Institut Universitaet Zuerich (Switzerland); Swiss Light Source PSI (Switzerland); Petrov, Vladimir [Physics Institute St Petersburg (Russian Federation); Patthey, Luc [Swiss Light Source PSI (Switzerland); Osterwalder, Juerg [Physik Institut Universitaet Zuerich (Switzerland)

    2009-07-01

    By a controllable change in the stoichiometry of the long range ordered mixed surface alloy (Bi/Pb/Sb)/Ag(111) the Rashba and Fermi energy can be tuned over a wide range. We show by spin and angle-resolved photoemission spectroscopy that the spin structure of the individual surface state bands remain unaffected despite the random intermixing of the adatoms. We further report on the observation of unconventional Fermi surface spin textures. These spin textures are found when the Fermi energy lies between the crossing point and the apex of the Rashba type Kramer's pair. The results will be discussed in the context of spin transport.

  15. Analytic model for low energy excitation states and phase transitions in spin-ice systems

    Science.gov (United States)

    López-Bara, F. I.; López-Aguilar, F.

    2017-04-01

    Low energy excitation states in magnetic structures of the so-called spin-ices are produced via spin flips among contiguous tetrahedra of their crystal structure. These spin flips generate entities which mimic magnetic dipoles in every two tetrahedra according to the dumbbell model. When the temperature increases, the spin-flip processes are transmitted in the lattice, generating so-called Dirac strings, which constitute structural entities that can present mimetic behavior similar to that of magnetic monopoles. In recent studies of both specific heat and ac magnetic susceptibility, two (even possibly three) phases have been shown to vary the temperature. The first of these phases presents a sharp peak in the specific heat and another phase transition occurs for increasing temperature whose peak is broader than that of the former phase. The sharp peak occurs when there are no free individual magnetic charges and temperature of the second phase transition coincides with the maximum proliferation of free deconfined magnetic charges. In the present paper, we propose a model for analyzing the low energy excitation many-body states of these spin-ice systems. We give analytical formulas for the internal energy, specific heat, entropy and their temperature evolution. We study the description of the possible global states via the nature and structure of their one-body components by means of the thermodynamic functions. Below 0.37 K, the Coulomb-like magnetic charge interaction can generate a phase transition to a condensation of pole–antipole pairs, possibly having Bose–Einstein structure which is responsible for the sharp peak of the first phase transition. When there are sufficient free positive and negative charges, the system tends to behave as a magnetic plasma, which implies the broader peak in the specific heat appearing at higher temperature than the sharper experimental peak.

  16. Generalized Surface Polaritons and their quantum spin Hall effect

    CERN Document Server

    Xu, Yadong; Chen, Huanyang

    2016-01-01

    Surface polaritons, e.g., surface plasmon polaritons, are invaluable tools in nanophotonics. However, considerable plasmon loss narrows the application regime of plasmonic devices. Here we reveal some general conditions for lossless surface polaritons to emerge at the interface of a gain and a loss media. The gain medium does not only compensate the energy loss, but also modifies surface wave oscillation mechanisms. A new type of surface polaritons induced by the sign switch of the imaginary part of the permittivity across the interface is discovered. The surface polaritons exhibit spin Hall effect due to spin-momentum locking and unique Berry phase. The spin Hall coefficient changes the sign across the parity-time symmetric limit and becomes quantized for perfect metal-dielectric interface and for dielectric-dielectric interface with very large permittivity contrast, carrying opposite topological numbers. Our study opens a new direction for manipulating light with surface polaritons in non-Hermitian optical ...

  17. Dimers on Surface Graphs and Spin Structures. I

    DEFF Research Database (Denmark)

    Cimasoni, David; Reshetikhin, Nicolai

    2007-01-01

    Partition functions for dimers on closed oriented surfaces are known to be alternating sums of Pfaffians of Kasteleyn matrices. In this paper, we obtain the formula for the coefficients in terms of discrete spin structures.......Partition functions for dimers on closed oriented surfaces are known to be alternating sums of Pfaffians of Kasteleyn matrices. In this paper, we obtain the formula for the coefficients in terms of discrete spin structures....

  18. Exciting Graphene Surface Plasmon Polaritons through Light and Sound Interplay

    KAUST Repository

    Farhat, Mohamed

    2013-12-05

    We propose a concept that allows for efficient excitation of surface plasmon spolaritons (SPPs) on a thin graphene sheet located on a substrate by an incident electromagnetic field. Elastic vibrations of the sheet, which are generated by a flexural wave, act as a grating that enables the electromagnetic field to couple to propagating graphene SPPs. This scheme permits fast on-off switching of the SPPs and dynamic tuning of their excitation frequency by adjusting the vibration frequency (grating period). Potential applications include single molecule detection and enhanced control of SPP trajectories via surface wave patterning of graphene metasurfaces. Analytical calculations and numerical experiments demonstrate the practical applicability of the proposed concept.

  19. Efficiency of local surface plasmon polariton excitation on ridges

    DEFF Research Database (Denmark)

    Radko, I.P.; Bozhevolnyi, S.I.; Brucoli, G.

    2008-01-01

    The issue of efficient local coupling of light into surface plasmon polariton (SPP) modes is an important concern in miniaturization of plasmonic components. Here we present experimental and numerical investigations of efficiency of local SPP excitation on gold ridges of rectangular profile...... positioned on a gold film. The excitation is accomplished by illuminating the metal surface normally with a focused laser beam. Wavelength dependence and dependence of the efficiency on geometrical parameters of ridges are examined. Using leakage radiation microscopy, the efficiency of ˜20% is demonstrated...

  20. Progress in Neutron Scattering Studies of Spin Excitations in High-Tc Cuprates

    Science.gov (United States)

    Fujita, Masaki; Hiraka, Haruhiro; Matsuda, Masaaki; Matsuura, Masato; Tranquada, John M.; Wakimoto, Shuichi; Xu, Guangyong; Yamada, Kazuyoshi

    2012-01-01

    Neutron scattering experiments continue to improve our knowledge of spin fluctuations in layered cuprates, excitations that are symptomatic of the electronic correlations underlying high-temperature superconductivity. Time-of-flight spectrometers, together with new and varied single crystal samples, have provided a more complete characterization of the magnetic energy spectrum and its variation with carrier concentration. While the spin excitations appear anomalous in comparison with simple model systems, there is clear consistency among a variety of cuprate families. Focusing initially on hole-doped systems, we review the nature of the magnetic spectrum, and variations in magnetic spectral weight with doping. We consider connections with the phenomena of charge and spin stripe order, and the potential generality of such correlations as suggested by studies of magnetic-field and impurity induced order. We contrast the behavior of the hole-doped systems with the trends found in the electron-doped superconductors. Returning to hole-doped cuprates, studies of translation-symmetry-preserving magnetic order are discussed, along with efforts to explore new systems. We conclude with a discussion of future challenges.

  1. Progress in Neutron Scattering Studies of Spin Excitations in High-T(c) Cuprates

    Energy Technology Data Exchange (ETDEWEB)

    Fujita M.; Tranquada J.; Hiraka, H.; Matsuda, M.; Matsuura, M.; Wakimoto, S.; Xu, G.; Yamada, K.

    2012-01-01

    Neutron scattering experiments continue to improve our knowledge of spin fluctuations in layered cuprates, excitations that are symptomatic of the electronic correlations underlying high-temperature superconductivity. Time-of-flight spectrometers, together with new and varied single crystal samples, have provided a more complete characterization of the magnetic energy spectrum and its variation with carrier concentration. While the spin excitations appear anomalous in comparison with simple model systems, there is clear consistency among a variety of cuprate families. Focusing initially on hole-doped systems, we review the nature of the magnetic spectrum, and variations in magnetic spectral weight with doping. We consider connections with the phenomena of charge and spin stripe order, and the potential generality of such correlations as suggested by studies of magnetic-field and impurity induced order. We contrast the behavior of the hole-doped systems with the trends found in the electron-doped superconductors. Returning to hole-doped cuprates, studies of translation-symmetry-preserving magnetic order are discussed, along with efforts to explore new systems. We conclude with a discussion of future challenges.

  2. Modeling Spin Fluctuations and Magnetic Excitations from Time-Dependent Density Functional Theory

    Science.gov (United States)

    Gorni, Tommaso; Timrov, Iurii; Dal Corso, Andrea; Baroni, Stefano

    Harnessing spin fluctuations and magnetic excitations in materials is key in many fields of technology, spanning from memory devices to information transfer and processing, to name but a few. A proper understanding of the interplay between collective and single-particle spin excitations is still lacking, and it is expected that first-principle simulations based on TDDFT may shed light on this interplay, as well as on the role of important effects such as relativistic ones and related magnetic anisotropies. All the numerical approaches proposed so far to tackle this problem are based on the computationally demanding solution of the Sternheimer equations for the response orbitals or the even more demanding solution of coupled Dyson equations for the spin and charge susceptibilities. The Liouville-Lanczos approach to TDDFT has already proven to be a valuable alternative, the most striking of its features being the avoidance of sums over unoccupied single-particle states and the frequency-independence of the main numerical bottleneck. In this work we present an extension of this methodology to magnetic systems and its implementation in the Quantum ESPRESSO distribution, together with a few preliminary results on the magnon dispersions in bulk Fe.

  3. Birefringence controlled room-temperature picosecond spin dynamics close to the threshold of vertical-cavity surface-emitting laser devices

    Science.gov (United States)

    Li, M. Y.; Jähme, H.; Soldat, H.; Gerhardt, N. C.; Hofmann, M. R.; Ackemann, T.

    2010-11-01

    We analyze the spin-induced circular polarization dynamics at the threshold of vertical-cavity surface-emitting lasers at room-temperature using a hybrid excitation combining electrically pumping without spin preference and spin-polarized optical injection. After a short pulse of spin-polarized excitation, fast oscillations of the circular polarization degree (CPD) are observed within the relaxation oscillations. A theoretical investigation of this behavior on the basis of a rate equation model shows that these fast oscillations of CPD could be suppressed by means of a reduction of the birefringence of the laser cavity.

  4. Topological honeycomb magnon Hall effect: A calculation of thermal Hall conductivity of magnetic spin excitations

    Science.gov (United States)

    Owerre, S. A.

    2016-07-01

    Quite recently, the magnon Hall effect of spin excitations has been observed experimentally on the kagome and pyrochlore lattices. The thermal Hall conductivity κxy changes sign as a function of magnetic field or temperature on the kagome lattice, and κxy changes sign upon reversing the sign of the magnetic field on the pyrochlore lattice. Motivated by these recent exciting experimental observations, we theoretically propose a simple realization of the magnon Hall effect in a two-band model on the honeycomb lattice. The magnon Hall effect of spin excitations arises in the usual way via the breaking of inversion symmetry of the lattice, however, by a next-nearest-neighbour Dzyaloshinsky-Moriya interaction. We find that κxy has a fixed sign for all parameter regimes considered. These results are in contrast to the Lieb, kagome, and pyrochlore lattices. We further show that the low-temperature dependence on the magnon Hall conductivity follows a T2 law, as opposed to the kagome and pyrochlore lattices. These results suggest an experimental procedure to measure thermal Hall conductivity within a class of 2D honeycomb quantum magnets and ultracold atoms trapped in a honeycomb optical lattice.

  5. Coupling of Spin and Orbital Excitations in the Iron-based Superconductor FeSe0.5Te0.5

    Energy Technology Data Exchange (ETDEWEB)

    Lee, S.H.; Xu, G.; Ku, W.; Wen, J.S.; Lee, C.C.: Katayama, N.; Xu, Z.J.; Ji, S.; Lin, Z.W.; Gu, G. D.; Yang, H.-B.; Johnson, P.D.; Pan, Z.-H.; Valla, T.; Fujita, M.; Sato, T.J.; Chang, S.; Yamada, K.; Tranquada, J.M.

    2010-06-14

    We present a combined analysis of neutron scattering and photoemission measurements on superconducting FeSe{sub 0.5}Te{sub 0.5}. The low-energy magnetic excitations disperse only in the direction transverse to the characteristic wave vector (1/2,0,0) whereas the electronic Fermi surface near (1/2,0,0) appears to consist of four incommensurate pockets. While the spin resonance occurs at an incommensurate wave vector compatible with nesting, neither spin-wave nor Fermi-surface-nesting models can describe the magnetic dispersion. We propose that a coupling of spin and orbital correlations is key to explaining this behavior. If correct, it follows that these nematic fluctuations are involved in the resonance and could be relevant to the pairing mechanism.

  6. Coupling of spin and orbital excitations in the iron-based superconductor FeSe0.5Te0.5

    Energy Technology Data Exchange (ETDEWEB)

    Lee, S.-H.; Xu, Guangyong; Ku, Wei; Wen, J.S.; Lee, C.C.; Katayama, N.; Xu, Z.J.; Ji, S.; Lin, Z.W.; Gu, G.D.; Yang, H.-B.; Johnson, Peter D.; Pan, Z.-H.; Valla, Tonica; Fujita, M.; Sato, T.J.; Chang, S.; Yamada, K.; Tranquada, John M.

    2010-06-14

    We present a combined analysis of neutron scattering and photoemission measurements on superconducting FeSe{sub 0.5} Te{sub 0.5} . The low-energy magnetic excitations disperse only in the direction transverse to the characteristic wave vector (1/2 ,0,0) whereas the electronic Fermi surface near (1/2 ,0,0) appears to consist of four incommensurate pockets. While the spin resonance occurs at an incommensurate wave vector compatible with nesting, neither spin-wave nor Fermi-surface-nesting models can describe the magnetic dispersion. We propose that a coupling of spin and orbital correlations is key to explaining this behavior. If correct, it follows that these nematic fluctuations are involved in the resonance and could be relevant to the pairing mechanism.

  7. Spin-wave mode profiles versus surface/interface conditions in ferromagnetic Fe/Ni layered composites

    CERN Document Server

    Krawczyk, M; Levy, J C S; Mercier, D

    2003-01-01

    Spin-wave excitations in ferromagnetic layered composite (AB centre dot centre dot centre dot BA; A and B being different homogeneous ferromagnetic materials) are analysed theoretically, by means of the transfer matrix approach. The properties of multilayer spin-wave mode profiles are discussed in relation to multilayer characteristics, such as the filling fraction and the exchange or magnetization contrast; also, surface spin pinning conditions and dipolar interactions are taken into account. The interface conditions are satisfied by introducing an effective exchange field expressed by interface gradients of the exchange constant and the magnetization. This approach provides an easy way to find frequencies and amplitudes of standing spin waves in the multilayer. The developed theory is applied to interpretation of spin wave resonance (SWR) spectra obtained experimentally by Chambers et al in two systems: a bilayer Fe/Ni and a trilayer Ni/Fe/Ni, in perpendicular (to the multilayer surface) configuration of th...

  8. The Binding Energy, Spin-Excitation Gap, and Charged Gap in the Boson-Fermion Model

    Institute of Scientific and Technical Information of China (English)

    YANG Kai-Hua; TIAN Guang-Shan; HAN Ru-Qi

    2003-01-01

    In this paper, by applying a simplified version of Lieb 's spin-refleetion-positivity method, which was recentlydeveloped by one of us [G.S. Tian and J.G. Wang, J. Phys. A: Math. Gen. 35 (2002) 941], we investigate some generalproperties of the boson-fermion Hamiltonian, which has been widely used as a phenomenological model to describe thereal-space pairing of electrons. On a mathematically rigorous basis, we prove that for either negative or positive couplingV, which represents the spontaneous decay and recombination process between boson and fermion in the model, thepairing energy of electrons is nonzero. Furthermore, we also show that the spin-excitation gap of the boson-fermionHamiltonian is always larger than its charged gap, as predicted by the pre-paired electron theory.

  9. Analysis of the broadband chaotic spin-wave excitations in an active ring oscillator based on a metalized ferrite film

    Science.gov (United States)

    Kondrashov, A. V.; Ustinov, A. B.; Kalinikos, B. A.; Demokritov, S. O.

    2016-11-01

    This paper reports the first experimental study of broadband chaotic nonlinear spin- wave excitations which is formed through development of four-wave parametric processes in active ring oscillator based on metallized ferrite film. We find that an increase in the oscillation power leads to Hopf bifurcations sequence. Monochromatic, periodic quasi-periodic and chaotic excitations are observed. Spectra of the chaotic excitations consist of series of chaotic bands separated well in frequency. Parameters of the chaotic attractors are discussed.

  10. Extremely confined gap surface-plasmon modes excited by electrons

    DEFF Research Database (Denmark)

    Raza, Søren; Stenger, Nicolas; Pors, Anders Lambertus

    2014-01-01

    High-spatial and energy resolution electron energy-loss spectroscopy (EELS) can be used for detailed characterization of localized and propagating surface-plasmon excitations in metal nanostructures, giving insight into fundamental physical phenomena and various plasmonic effects. Here, applying...

  11. Localization of optical excitations on random surfaces: SNOM studies

    DEFF Research Database (Denmark)

    Bozhevolnyi, Sergey I.

    1999-01-01

    Localization of optical excitations on nanostructured metal surfaces and fractal colloid silver aggregates are studied by using a scanning near-field optical microscope (SNOM). The SNOM images obtained in both configurations exhibit spatially localized (within 150 to 250 nm) light intensity...

  12. Femtosecond switching of magnetism via strongly correlated spin-charge quantum excitations.

    Science.gov (United States)

    Li, Tianqi; Patz, Aaron; Mouchliadis, Leonidas; Yan, Jiaqiang; Lograsso, Thomas A; Perakis, Ilias E; Wang, Jigang

    2013-04-04

    The technological demand to push the gigahertz (10(9) hertz) switching speed limit of today's magnetic memory and logic devices into the terahertz (10(12) hertz) regime underlies the entire field of spin-electronics and integrated multi-functional devices. This challenge is met by all-optical magnetic switching based on coherent spin manipulation. By analogy to femtosecond chemistry and photosynthetic dynamics--in which photoproducts of chemical and biochemical reactions can be influenced by creating suitable superpositions of molecular states--femtosecond-laser-excited coherence between electronic states can switch magnetic order by 'suddenly' breaking the delicate balance between competing phases of correlated materials: for example, manganites exhibiting colossal magneto-resistance suitable for applications. Here we show femtosecond (10(-15) seconds) photo-induced switching from antiferromagnetic to ferromagnetic ordering in Pr0.7Ca0.3MnO3, by observing the establishment (within about 120 femtoseconds) of a huge temperature-dependent magnetization with photo-excitation threshold behaviour absent in the optical reflectivity. The development of ferromagnetic correlations during the femtosecond laser pulse reveals an initial quantum coherent regime of magnetism, distinguished from the picosecond (10(-12) seconds) lattice-heating regime characterized by phase separation without threshold behaviour. Our simulations reproduce the nonlinear femtosecond spin generation and underpin fast quantum spin-flip fluctuations correlated with coherent superpositions of electronic states to initiate local ferromagnetic correlations. These results merge two fields, femtosecond magnetism in metals and band insulators, and non-equilibrium phase transitions of strongly correlated electrons, in which local interactions exceeding the kinetic energy produce a complex balance of competing orders.

  13. Spin polarization asymmetry at the surface of chromia

    Science.gov (United States)

    Cao, Shi; Zhang, Xin; Wu, Ning; N'Diaye, A. T.; Chen, G.; Schmid, A. K.; Chen, Xumin; Echtenkamp, W.; Enders, A.; Binek, Ch; Dowben, P. A.

    2014-07-01

    We demonstrate boundary spin polarization at the surface of a Cr2O3 single crystal using spin-polarized low-energy electron microscopy (SPLEEM), complementing prior spin polarized photoemission, spin polarized inverse photoemission, and x-ray magnetic circular dichroism photoemission electron microscopy measurements. This work shows that placing a Cr2O3 single crystal into a single domain state will result in net Cr2O3 spin polarization at the boundary, even in the presence of a gold overlayer. There are indications that the SPLEEM contrast for the two polarization states may be different, consistent with scanning tunneling microscopy spectroscopy results obtained from ultrathin films of Cr2O3.

  14. Odd-spin yrast states as multiple quadrupole-phonon excitations

    CERN Document Server

    Pietralla, N; Otsuka, T; Casten, R F

    1995-01-01

    The wavefunctions of the lowest odd spin positive parity yrast states in the IBA are shown to be nearly pure multiple quadrupole-phonon excitations even outside the three dynamical symmetries. The empirical data for collective nuclei with 30 < Z < 80 confirm these predictions. The quadrupole-phonon purity of the 2^+_1 state can be measured from E2-branching ratios of the 3^+_1 state. These data show a high correlation to the 2^+_1 Q-phonon purity deduced from the E2-decay of 2^+ states.

  15. The surface spin polarization of Co-based Heusler alloys

    Energy Technology Data Exchange (ETDEWEB)

    Fetzer, Roman; Wuestenberg, Jan-Peter; Neuschwander, Sabine; Aeschlimann, Martin; Cinchetti, Mirko [University of Kaiserslautern (Germany). Department of Physics and Research Center OPTIMAS; Jourdan, Martin; Herbort, Christian; Vilanova Vidal, Enrique; Jakob, Gerhard [University of Mainz (Germany). Institute of Physics

    2010-07-01

    Co-based Heusler alloys belong mainly to the family of half-metallic ferromagnets (HMFs). The predicted full spin polarization at the Fermi level due to the minority spin band gap makes this class of materials highly interesting for application in the field of spintronics. Thus, the characterization of the surface of Co-based Heusler compounds is extremely relevant for understanding and improving the performance of Heusler-based spintronics devices, like tunnel-magnetoresistance (TMR) junctions. Using Auger electron spectroscopy (AES) and low energy spin polarized electron photoemission, we systematically studied the correlation between chemical composition and spin polarisation of the surface. For various Co-based Heusler alloys, e.g. Co{sub 2}CrAl, Co{sub 2}MnAl and Co{sub 2}FeGa{sub 0.5}Ge{sub 0.5}, we found different degrees of spin-polarization at the very surface region. Reasons for the distinct deviation from the predicted 100% spin polarization and the dependence on the specific surface preparation procedure are discussed.

  16. Excitation of a surface plasmon with an elastomeric grating

    Science.gov (United States)

    Kocabas, A.; Dâna, A.; Aydinli, A.

    2006-07-01

    We report on a new method to excite surface plasmon polaritons on a thin metal slab surface using an elastomeric grating which is fabricated by replica molding technique. The grating is placed on the metal surface which creates a periodic perturbation on the surface matching the momentum of the incident light to that of the surface plasmon. The conformal contact between the metal surface and the elastomeric grating changes the dielectric medium periodically and allows the observation of an effective surface plasmon polariton at the metal-air and metal-polymer interfaces of the grating. To clarify the nature of the observed plasmon, comparison of the elastomeric grating with elastomeric slabs was performed with the attenuated total reflection method.

  17. Multiple photon excited SF6 interaction with silicon surfaces

    Science.gov (United States)

    Chuang, T. J.

    1981-01-01

    Infrared laser induced SF6-silicon interactions have been studied and the surface reaction yields have been determined as a function of the laser frequency, the laser intensity, and the gas pressure in both perpendicular and parallel beam incidences on the solid surfaces. The results clearly show that vibrationally excited SF6 molecules promoted by CO2 laser pulses are very reactive to silicon, particularly when the solid is simultaneously exposed to the intense ir radiation. The laser excitation of the Si substrate alone cannot cause the heterogeneous reaction to occur. The present gas-solid system thus provides an example which clearly establishes the direct correlation between surface reactivity and vibrational activation. Additional experimental measurements also demonstrate that the thermal fluorine atoms generated by SF6 multiple photon dissociation at high laser intensities can react with silicon to form volatile product. The study thus provides further insight into the silicon-fluorine reaction dynamics.

  18. Asymmetric excitation of surface plasmons by dark mode coupling.

    Science.gov (United States)

    Zhang, Xueqian; Xu, Quan; Li, Quan; Xu, Yuehong; Gu, Jianqiang; Tian, Zhen; Ouyang, Chunmei; Liu, Yongmin; Zhang, Shuang; Zhang, Xixiang; Han, Jiaguang; Zhang, Weili

    2016-02-01

    Control over surface plasmons (SPs) is essential in a variety of cutting-edge applications, such as highly integrated photonic signal processing systems, deep-subwavelength lasing, high-resolution imaging, and ultrasensitive biomedical detection. Recently, asymmetric excitation of SPs has attracted enormous interest. In free space, the analog of electromagnetically induced transparency (EIT) in metamaterials has been widely investigated to uniquely manipulate the electromagnetic waves. In the near field, we show that the dark mode coupling mechanism of the classical EIT effect enables an exotic and straightforward excitation of SPs in a metasurface system. This leads to not only resonant excitation of asymmetric SPs but also controllable exotic SP focusing by the use of the Huygens-Fresnel principle. Our experimental findings manifest the potential of developing plasmonic metadevices with unique functionalities.

  19. Asymmetric excitation of surface plasmons by dark mode coupling

    KAUST Repository

    Zhang, X.

    2016-02-19

    Control over surface plasmons (SPs) is essential in a variety of cutting-edge applications, such as highly integrated photonic signal processing systems, deep-subwavelength lasing, high-resolution imaging, and ultrasensitive biomedical detection. Recently, asymmetric excitation of SPs has attracted enormous interest. In free space, the analog of electromagnetically induced transparency (EIT) in metamaterials has been widely investigated to uniquely manipulate the electromagnetic waves. In the near field, we show that the dark mode coupling mechanism of the classical EIT effect enables an exotic and straightforward excitation of SPs in a metasurface system. This leads to not only resonant excitation of asymmetric SPs but also controllable exotic SP focusing by the use of the Huygens-Fresnel principle. Our experimental findings manifest the potential of developing plasmonic metadevices with unique functionalities.

  20. Dimerization process and elementary excitations in spin-Peierls chains coupled by frustrated interactions

    Energy Technology Data Exchange (ETDEWEB)

    Mastrogiuseppe, D; Gazza, C; Dobry, A [Facultad de Ciencias Exactas IngenierIa y Agrimensura, Universidad Nacional de Rosario and Instituto de Fisica Rosario, Boulevard 27 de Febrero 210 bis, 2000 Rosario (Argentina)], E-mail: dmastro@ifir.edu.ar

    2008-04-02

    We consider the ground state and the elementary excitations of an array of spin-Peierls chains coupled by elastic and magnetic interactions. It is expected that the effect of the magnetic interchain coupling will be to reduce the dimerization amplitude and that of the elastic coupling will be to confine the spin one-half solitons corresponding to each isolated chain. We show that this is the case when these interactions are not frustrated. On the other hand, in the frustrated case we show that the amplitude of dimerization in the ground state is independent of the strength of the interchain magnetic interaction in a broad range of values of this parameter. We also show that free solitons could be the elementary excitations when only nearest neighbour interactions are considered. The case of an elastic interchain coupling is analysed on a general energetic consideration. To study the effect of the magnetic interchain interaction the problem is simplified to a two-leg ladder, which is solved using density matrix renormalization group (DMRG) calculations. We show that the deconfinement mechanism is effective even with a significantly strong antiferromagnetic interchain coupling.

  1. Self-excitation of Rydberg atoms at a metal surface

    Science.gov (United States)

    Bordo, V. G.

    2017-08-01

    The novel effect of self-excitation of an atomic beam propagating above a metal surface is predicted and a theory is developed. Its underlying mechanism is positive feedback provided by the reflective surface for the atomic polarization. Under certain conditions the atomic beam flying in the near field of the metal surface acts as an active device that supports sustained atomic dipole oscillations, which generate, in their turn, an electromagnetic field. This phenomenon does not exploit stimulated emission and therefore does not require population inversion in atoms. An experiment with Rydberg atoms in which this effect should be most pronounced is proposed and the necessary estimates are given.

  2. Self-excitation of Rydberg atoms at a metal surface

    DEFF Research Database (Denmark)

    Bordo, Vladimir

    2017-01-01

    The novel effect of self-excitation of an atomic beam propagating above a metal surface is predicted and a theory is developed. Its underlying mechanism is positive feedback provided by the reflective surface for the atomic polarization. Under certain conditions the atomic beam flying in the near...... field of the metal surface acts as an active device that supports sustained atomic dipole oscillations, which generate, in their turn, an electromagnetic field. This phenomenon does not exploit stimulated emission and therefore does not require population inversion in atoms. An experiment with Rydberg...... atoms in which this effect should be most pronounced is proposed and the necessary estimates are given....

  3. Excitation of Self-Localized Spin-Wave Bullets by Spin-Polarized Current in In-Plane Magnetized Magnetic Nano-Contacts: A Micromagnetic Study

    Science.gov (United States)

    2007-10-08

    Melkov,3 Vasil Tiberkevich,4 and Andrei N. Slavin4 1Dipartimento di Fisica della Materia e Tecnologie Fisiche Avanzate, University of Messina...nanocontact. In Eq. 1, the unit vector p defining the spin-polarization direction is parallel to the direction ez of the in-plane external magnetic field...linear theory,3 the propagating spin- wave mode excited at the threshold is a cylindrical spin- wave with the wave vector kL=1.2/Rc and frequency L

  4. Spin relaxation and the Elliott-Yafet parameter in W(001) ultrathin films: Surface states, anisotropy, and oscillation effects

    Science.gov (United States)

    Long, Nguyen H.; Mavropoulos, Phivos; Zimmermann, Bernd; Heers, Swantje; Bauer, David S. G.; Blügel, Stefan; Mokrousov, Yuriy

    2013-06-01

    Using first-principles methods based on density-functional theory, we investigate the spin relaxation in W(001) ultrathin films. Within the framework of the Elliott-Yafet theory, we calculate the spin mixing of the Bloch states and we explicitly consider spin-flip scattering off self-adatoms. At small film thicknesses, we find an oscillatory behavior of the spin-mixing parameter and relaxation rate as a function of the film thickness, which we trace back to surface-state properties. We also analyze the Rashba effect experienced by the surface states and discuss its influence on the spin relaxation. Finally, we calculate the anisotropy of the spin-relaxation rate with respect to the polarization direction of the excited spin population relative to the crystallographic axes of the film. We find that the spin-relaxation rate can increase by as much as 27% when the spin polarization is directed out of plane, compared to the case when it is in plane. Our calculations are based on the multiple-scattering formalism of the Korringa-Kohn-Rostoker Green-function method.

  5. Dynamic nuclear spin polarization in the resonant laser excitation of an InGaAs quantum dot.

    Science.gov (United States)

    Högele, A; Kroner, M; Latta, C; Claassen, M; Carusotto, I; Bulutay, C; Imamoglu, A

    2012-05-11

    Resonant optical excitation of lowest-energy excitonic transitions in self-assembled quantum dots leads to nuclear spin polarization that is qualitatively different from the well-known optical orientation phenomena. By carrying out a comprehensive set of experiments, we demonstrate that nuclear spin polarization manifests itself in quantum dots subjected to finite external magnetic field as locking of the higher energy Zeeman transition to the driving laser field, as well as the avoidance of the resonance condition for the lower energy Zeeman branch. We interpret our findings on the basis of dynamic nuclear spin polarization originating from noncollinear hyperfine interaction and find excellent agreement between experiment and theory. Our results provide evidence for the significance of noncollinear hyperfine processes not only for nuclear spin diffusion and decay, but also for buildup dynamics of nuclear spin polarization in a coupled electron-nuclear spin system.

  6. External magnetic field dependent shift of superparamagnetic blocking temperature due to core/surface disordered spin interactions

    Science.gov (United States)

    Lee, Kwan; Jang, Jung-tak; Nakano, Hiroshi; Nakagawa, Shigeki; Paek, Sun Ha; Bae, Seongtae

    2017-02-01

    Although the blocking temperature of superparamagnetic nanoparticles (SPNPs) is crucial for various spintronics and biomedical applications, the precise determination of the blocking temperature is still not clear. Here, we present ‘intrinsic’ and ‘extrinsic’ characteristics of the blocking temperature in SPNP systems. In zero-field-cooled/field-cooled (ZFC-FC) curves, there was no shift of ‘intrinsic blocking temperature’ at different applied external (excitation) magnetic fields. However, ‘extrinsic blocking temperature’ shift is clearly dependent on the external (excitation) magnetic field. According to our newly proposed physical model, the ‘intermediate spin layer’ located between the core and surface disordered spin layers is primarily responsible for the physical nature of the shift of extrinsic blocking temperature. Our new findings offer possibilities for characterizing the thermally induced physical properties of SPNPs. Furthermore, these findings provide a new empirical approach to indirectly estimate the qualitative degree of the disordered surface spin status in SPNPs.

  7. Polarization controlled directional excitation of Bloch surface waves (Conference Presentation)

    Science.gov (United States)

    Kovalevich, Tatiana; Boyer, Philippe; Bernal, Maria-Pilar; Kim, Myun-Sik; Herzig, Hans Peter; Grosjean, Thierry

    2016-09-01

    Bloch surface waves (BSWs) are electromagnetic surface waves which can be excited at the interface between periodic dielectric multilayer and a surrounding medium. In comparison with surface plasmon polaritons these surface states perform high quality factor due to low loss characteristics of dielectric materials and can be exited both by TE and TM polarized light. A platform consisting of periodic stacks of alternative SiO2 and Si3N4 layers is designed and fabricated to work at the wavelength of 1.55 µm. The platform has an application in sensing and in integrated optics domain. A standard way of BSW excitation is coupling via Kretschmann configuration, but in this work we investigate a grating coupling of BSWs. Grating parameters are analytically and numerically optimized by RCWA and FDTD methods in order to obtain the best coupling conditions. The light is launched orthogonally to the surface of the photonic crystal and the grating. Due to a special grating configuration we demonstrate directionality of the BSW propagation depending on polarization of the incident light. The structure was experimentally realized on the surface of the photonic crystal by FIB milling. Experimental results are in a good agreement with a theory. The investigated configuration can be successfully used as a BSW launcher in on-chip all-optical integrated systems and work as a surface wave switch or modulator.

  8. On the influence of soft crystal field excitations on the spectrum of spin excitations in CeNiSn-type Kondo lattices

    Energy Technology Data Exchange (ETDEWEB)

    Kagan, Yu.; Kikoin, K.A.; Mishchenko, A.S. [RRC Kurchatov Inst., Moscow (Russian Federation). Super Conductivity and Solid State

    1997-02-01

    On the grounds of the microscopic theory of heavy-fermion spin liquids a novel description of low-energy excitation spectra in CeNiSn and related compounds is offered. The anomalous properties of orthorhombic CeNiSn and related materials are explained by the interplay between the fermi-type spinon excitations with the energy scale T{sup *} {approx} T{sub K} and the one-site crystal field excitations with the energy {Delta}{sub CF} < T{sup *}. The theory gives both quantitative and qualitative description of inelastic neutron scattering spectra and low-temperature thermodynamics. It resolves also the apparent contradiction between metallic conductivity and gap-wise behavior of thermodynamic properties and spin response at low temperatures. (orig.). 8 refs.

  9. Spin-excitations of the quantum Hall ferromagnet of composite fermions

    Science.gov (United States)

    Doretto, R. L.; Goerbig, M. O.; Lederer, P.; Caldeira, A. O.; Smith, C. Morais

    2005-07-01

    The spin excitations of a fractional quantum Hall system are evaluated within a bosonization approach. In a first step, we generalize Murthy and Shankar’s Hamiltonian theory of the fractional quantum Hall effect to the case of composite fermions with an extra discrete degree of freedom. Here, we mainly investigate the spin degrees of freedom, but the proposed formalism may be useful also in the study of bilayer quantum-Hall systems, where the layer index may formally be treated as an isospin. In a second step, we apply a bosonization scheme, recently developed for the study of the two-dimensional electron gas, to the interacting composite-fermion Hamiltonian. The dispersion of the bosons, which represent quasiparticle-quasihole excitations, is analytically evaluated for fractional quantum Hall systems at ν=1/3 and ν=1/5 . The finite width of the two-dimensional electron gas is also taken into account explicitly. Furthermore, we consider the interacting bosonic model and calculate the lowest-energy state for two bosons. In addition to a continuum describing scattering states, we find a bound-state of two bosons. This state is interpreted as a pair excitation, which consists of a skyrmion of composite fermions and an antiskyrmion of composite fermions. The dispersion relation of the two-boson state is evaluated for ν=1/3 and ν=1/5 . Finally, we show that our theory provides the microscopic basis for a phenomenological nonlinear σ model for studying the skyrmion of composite fermions.

  10. Surface spin-electron acoustic waves in magnetically ordered metals

    CERN Document Server

    Andreev, Pavel A

    2015-01-01

    Degenerate plasmas with motionless ions show existence of three surface waves: the Langmuir wave, the electromagnetic wave, and the zeroth sound. Applying the separated spin evolution quantum hydrodynamics to half-space plasma we demonstrate the existence of the surface spin-electron acoustic wave (SSEAW). We study dispersion of the SSEAW. We show that there is hybridization between the surface Langmuir wave and the SSEAW at rather small spin polarization. In the hybridization area the dispersion branches are located close to each other. In this area there is a strong interaction between these waves leading to the energy exchange. Consequently, generating the Langmuir waves with the frequencies close to hybridization area we can generate the SSEAWs. Thus, we report a method of creation of the SEAWs.

  11. Dimers on surface graphs and spin structures. II

    DEFF Research Database (Denmark)

    Cimasoni, David; Reshetikhin, Nicolai

    2009-01-01

    In a previous paper [3], we showed how certain orientations of the edges of a graph Γ embedded in a closed oriented surface Σ can be understood as discrete spin structures on Σ. We then used this correspondence to give a geometric proof of the Pfaffian formula for the partition function of the di......In a previous paper [3], we showed how certain orientations of the edges of a graph Γ embedded in a closed oriented surface Σ can be understood as discrete spin structures on Σ. We then used this correspondence to give a geometric proof of the Pfaffian formula for the partition function...... of the dimer model on Γ. In the present article, we generalize these results to the case of compact oriented surfaces with boundary. We also show how the operations of cutting and gluing act on discrete spin structures and how they change the partition function. These operations allow to reformulate the dimer...

  12. Investigation of Surface Magnetic Noise by Shallow Spins in Diamond

    OpenAIRE

    2014-01-01

    We present measurements of spin relaxation times (T1, T1ρ, T2) on very shallow (≲5  nm) nitrogen-vacancy centers in high-purity diamond single crystals. We find a reduction of spin relaxation times up to 30 times compared to bulk values, indicating the presence of ubiquitous magnetic impurities associated with the surface. Our measurements yield a density of 0.01–0.1μB/nm2 and a characteristic correlation time of 0.28(3) ns of surface states, with little variation between samples and chemical...

  13. Semi classical description of isotropic Non-Heisenberg magnets for spin S=3/2 and linear quadrupole excitation dynamics

    Directory of Open Access Journals (Sweden)

    Y Yousefi

    2012-09-01

    Full Text Available  In this paper, a system with spin S=3/2 with general isotropic nearest neighbor exchange within a mean field approximation possess is discnssed. We derive equations describing non-Heisenberg isotropic model using coherent states of SU(4 group in real parameters and then obtain dispersion equations of spin wave of dipole and quadrupole branches for a small linear excitation from the ground state.

  14. Inelastic neutron scattering study of spin excitations in the superconducting state of high temperature superconductors; Etude par diffusion inelastique de neutrons des excitations de spin dans la phase supraconductrice des supraconducteurs a haute temperature

    Energy Technology Data Exchange (ETDEWEB)

    Sidis, Y.; Pailhes, St.; Fauque, B.; Bourges, Ph. [CEA Saclay, Lab. Leon Brillouin, CNRS, 91 - Gif-sur-Yvette (France); Hinkov, V.; Ulrich, C.; Keimer, B. [Max-Planck-Institut fur Fertkorperforschung, Stuttgart (Germany); Capogna, L.; Ivanov, A. [Institut Laue-Langevin, 38 - Grenoble (France); Regnault, L.P. [CEA Grenoble, Dept. de Recherche Fondamentale sur la Matiere Condensee, 38 (France)

    2007-09-15

    Inelastic neutron scattering is a powerful technique that can measure magnetic correlations in a large momentum and energy range. In strongly correlated electronic systems, where spin, orbital, lattice and charge degrees of freedom are entangled, it is currently used to study the magnetic properties and shed light on their role in the appearance of the exotic electronic properties, such as unconventional superconductivity. In this article, we focus on the observation by inelastic neutron scattering technique of unconventional spin triplet collective modes in the superconducting state of high temperature superconducting cuprates and its interplay with anomalies in the charge excitation spectrum. The triplet spin mode is interpreted as a spin exciton, within a spin band model. Alternative scenarios based on localized or dual (itinerant localized) models are also mentioned. (authors)

  15. Nuclear response theory for spin-isospin excitations in a relativistic quasiparticle-phonon coupling framework

    CERN Document Server

    Robin, Caroline

    2016-01-01

    A new theoretical approach to spin-isospin excitations in open-shell nuclei is presented. The developed method is based on the relativistic meson-exchange nuclear Lagrangian of Quantum Hadrodynamics and extends the response theory for superfluid nuclear systems beyond relativistic quasiparticle random phase approximation in the proton-neutron channel (pn-RQRPA). The coupling between quasiparticle degrees of freedom and collective vibrations (phonons) introduces a time-dependent effective interaction, in addition to the exchange of pion and $\\rho$-meson taken into account without retardation. The time-dependent contributions are treated in the resonant time-blocking approximation, in analogy to previously developed relativistic quasiparticle time blocking approximation (RQTBA) in the neutral (non-isospin-flip) channel. The new method is called proton-neutron RQTBA (pn-RQTBA) and applied to Gamow-Teller resonance in a chain of neutron-rich Nickel isotopes $^{68-78}$Ni. A strong fragmentation of the resonance al...

  16. Adaptive Dynamic Surface Control for Generator Excitation Control System

    Directory of Open Access Journals (Sweden)

    Zhang Xiu-yu

    2014-01-01

    Full Text Available For the generator excitation control system which is equipped with static var compensator (SVC and unknown parameters, a novel adaptive dynamic surface control scheme is proposed based on neural network and tracking error transformed function with the following features: (1 the transformation of the excitation generator model to the linear systems is omitted; (2 the prespecified performance of the tracking error can be guaranteed by combining with the tracking error transformed function; (3 the computational burden is greatly reduced by estimating the norm of the weighted vector of neural network instead of the weighted vector itself; therefore, it is more suitable for the real time control; and (4 the explosion of complicity problem inherent in the backstepping control can be eliminated. It is proved that the new scheme can make the system semiglobally uniformly ultimately bounded. Simulation results show the effectiveness of this control scheme.

  17. Excitation of surface plasmons at the boundary of overdense plasma

    Institute of Scientific and Technical Information of China (English)

    Wang Liang; Cao Jin-Xiang; Wang Yan; Niu Tian-Ye; Liu Lei; Lü You

    2008-01-01

    The excitation of surface plasmons (SPs) with a strip grating at the boundary of an unmagnetized overdense plasma has been investigated theoretically and experimentally. An incident electromagnetic radiation was p-polarized at the frequency of 5 GHz. Experiments showed that when the plasma density was four times higher than the critical density with the grating present, and the SPs could be excited at the boundary of the overdense plasma. Contribution of the glass layer in the formation of the SP dispersion relation was examined. When the incident electromagnetic radiation was coupled into SPs the coupling order with the effective permittivity was simulated qualitatively. We find that the existence of SPs at the boundary of overdense plasma indicates that the reflection coefficient of the incident electromagnetic radiation reaches its minimum and even becomes total absorption. In this work the plasma density was diagnosed by a Langmuir double probe.

  18. T1 ρ-weighted MRI using a surface coil to transmit spin-lock pulses

    Science.gov (United States)

    Borthakur, Arijitt; Charagundla, Sridhar R.; Wheaton, Andrew; Reddy, Ravinder

    2004-04-01

    T1 ρ-weighted MRI is a novel basis for generating tissue contrast. However, it suffers from sensitivity to B1 inhomogeneity. First, excitation with a spatially varying B1 causes flip-angle artifacts and second, spin locking with an inhomogeneous B1 results in non-uniform T1 ρ contrast. In this study, we overcome the former complication with a specially designed spin-locking pulse sequence and we successfully obtain T1 ρ-weighted images with a surface coil. In this pulse sequence, the spin-lock pulse was divided into segments of equal duration and alternating phase. This "self-compensating" T1 ρ-preparatory pulse sequence was analyzed and the effect of an inhomogeneous B1 field was simulated using the Bloch equations. T1 ρ-weighted MR images of a phantom and a human knee joint in vivo were obtained on a clinical scanner with a surface coil to demonstrate the utility of the pulse sequence. The self-compensating T1 ρ-prepared pulses sequence resulted in substantially reduced image artifacts compared to the conventional, single-phase spin-lock pulse.

  19. Unidirectional propagation of magnetostatic surface spin waves at a magnetic film surface

    Energy Technology Data Exchange (ETDEWEB)

    Wong, Kin L.; Bao, Mingqiang, E-mail: mingqiangbao@gmail.com, E-mail: caross@mit.edu; Lin, Yen-Ting; Wang, Kang L. [Department of Electrical Engineering, University of California, Los Angeles, Los Angeles, California 90095 (United States); Bi, Lei [Department of Materials Science and Engineering, Massachusetts Institute of Technology, Cambridge, Massachusetts 02139 (United States); State Key Laboratory of Electronic Thin Films and Integrated Devices, University of Electronic Science and Technology of China, Chengdu 610054 (China); Wen, Qiye; Zhang, Huaiwu [State Key Laboratory of Electronic Thin Films and Integrated Devices, University of Electronic Science and Technology of China, Chengdu 610054 (China); Chatelon, Jean Pierre [Univerisité de Saint-Etienne, Université de Lyon, LT2C, 25 rue du Docteur Rémy Annino, 42000 Saint-Etienne (France); Ross, C. A., E-mail: mingqiangbao@gmail.com, E-mail: caross@mit.edu [Department of Materials Science and Engineering, Massachusetts Institute of Technology, Cambridge, Massachusetts 02139 (United States)

    2014-12-08

    An analytical expression for the amplitudes of magnetostatic surface spin waves (MSSWs) propagating in opposite directions at a magnetic film surface is presented. This shows that for a given magnetic field H, it is forbidden for an independent MSSW to propagate along the direction of −H{sup →}×n{sup →}, where n{sup →} is the surface normal. This unidirectional propagation property is confirmed by experiments with both permalloy and yttrium iron garnet films of different film thicknesses, and has implications in the design of spin-wave devices such as isolators and spin-wave diodes.

  20. Surface-step defect in three-dimensional topological insulators: Electric manipulation of spin and quantum spin Hall effect

    Science.gov (United States)

    Zhou, Yan-Feng; Guo, Ai-Min; Sun, Qing-Feng

    2016-08-01

    We study the influence of a step defect on surface states in three-dimensional topological insulators subject to a perpendicular magnetic field. By calculating the energy spectrum of the surface states, we find that Landau levels (LLs) can form on flat regions of the surface and are distant from the step defect, and several subbands emerge at the side surface of the step defect. The subband which connects to the two zeroth LLs is spin polarized and chiral. In particular, when the electron transports along the side surface, the electron spin direction can be manipulated arbitrarily by gate voltage. Also, no reflection occurs even if the electron spin direction is changed. This provides a fascinating avenue to control the electron spin easily and coherently. In addition, regarding the subbands with a high LL index, there exist spin-momentum locking helical states and the quantum spin Hall effect can appear.

  1. Transition from three-dimensional anisotropic spin excitations to two-dimensional spin excitations by electron doping the FeAs-based BaFe1.96Ni0.04As2 superconductor.

    Science.gov (United States)

    Harriger, Leland W; Schneidewind, Astrid; Li, Shiliang; Zhao, Jun; Li, Zhengcai; Lu, Wei; Dong, Xiaoli; Zhou, Fang; Zhao, Zhongxian; Hu, Jiangping; Dai, Pengcheng

    2009-08-21

    We use neutron scattering to study the effect of electron doping on the structural or magnetic order in BaFe2As2. In the undoped state, BaFe2As2 exhibits simultaneous structural and magnetic phase transitions below 143 K. Upon electron doping to form BaFe1.96Ni0.04As2, the system first displays the lattice distortion near approximately 97 K, and then orders antiferromagnetically at 91 K before developing weak superconductivity below approximately 15 K. The effect of electron doping is to reduce the c-axis exchange coupling in BaFe2As2 and induce quasi-two-dimensional (2D) spin excitations. These results suggest that the transition from 3D spin waves to quasi-2D spin excitations by electron doping is important for the separated structural and magnetic phase transitions in iron arsenides.

  2. Surface and Size Effects in Spin-Crossover Nanocrystals

    Science.gov (United States)

    Gudyma, Iurii; Ivashko, Victor; Bobák, Andrej

    2017-02-01

    We perform Monte Carlo simulations to analyze the surface and size effects in spin-crossover nanocrystals using an Ising-like model including surface and core intermolecular interactions. The consequences of downsizing effect on the transition temperature and the width of hysteresis as finger of the system cooperativity are discussed. The critical temperature is calculated using the real-space renormalization method. The obtained results are in agreement with the experimental data.

  3. Stern Gerlach spin filter using surface acoustic waves

    Science.gov (United States)

    Santos, Paulo V.; Nitta, Junsaku; Ploog, Klaus H.

    2004-12-01

    We propose the ambipolar carrier transport by surface acoustic waves (SAWs) in a semiconductor quantum well (QW) for the realization of the Stern-Gerlach (SG) experiment in the solid phase. The well-defined and very low carrier velocity in the moving SAW field leads to a large deflection angle and thus to efficient spin separation, even for the weak field gradients and short (μm-long) interaction lengths that can be produced by micromagnets. The feasibility of a SG spin filter is discussed for different QW materials.

  4. Current-induced spin polarization on a Pt surface: A new approach using spin-polarized positron annihilation spectroscopy

    Energy Technology Data Exchange (ETDEWEB)

    Kawasuso, A., E-mail: kawasuso.atsuo@jaea.go.jp [Advanced Science Research Center, Japan Atomic Energy Agency, 1233 Watanuki, Takasaki, Gunma 370-1292 (Japan); Fukaya, Y.; Maekawa, M.; Zhang, H. [Advanced Science Research Center, Japan Atomic Energy Agency, 1233 Watanuki, Takasaki, Gunma 370-1292 (Japan); Seki, T.; Yoshino, T.; Saitoh, E.; Takanashi, K. [Institute for Materials Research, Tohoku University, 2-1-1 Katahira, Aoba-ku, Sendai 980-8577 (Japan)

    2013-09-15

    Transversely spin-polarized positrons were injected near Pt and Au surfaces under an applied electric current. The three-photon annihilation of spin-triplet positronium, which was emitted from the surfaces into vacuum, was observed. When the positron spin polarization was perpendicular to the current direction, the maximum asymmetry of the three-photon annihilation intensity was observed upon current reversal for the Pt surfaces, whereas it was significantly reduced for the Au surface. The experimental results suggest that electrons near the Pt surfaces were in-plane and transversely spin-polarized with respect to the direction of the electric current. The maximum electron spin polarization was estimated to be more than 0.01 (1%). - Highlights: • Annihilation probability of positronium emitted from the Pt surface into the vacuum under direct current exhibited asymmetry upon current reversal. • The maximum asymmetry appeared when positron spin polarization and the direct current were perpendicular to each other. • Electrons near the Pt surfaces were in-plane and transversely spin-polarized with respect to the direction of the electric current. • Spin-polarized positronium annihilation provides a unique tool for investigating spin polarization on metal surfaces.

  5. Evaluation of excitation energy and spin in fission fragments using the statistical model, and the FIPPS project

    Directory of Open Access Journals (Sweden)

    Sage C.

    2013-03-01

    Full Text Available We review the statistical model and its application for the process of nuclear fission. The expressions for excitation energy and spin distributions for the individual fission fragments are given. We will finally emphasize the importance of measuring prompt gamma decay to further test the statistical model in nuclear fission with the FIPPS project.

  6. Adding a spin to Kerker's condition: arbitrary scattering direction tuning of nano-antennas with designed excitation

    CERN Document Server

    Wei, Lei; Urbach, H Paul

    2016-01-01

    A way to control the scattering to any direction in a plane over a broad wavelength range is proposed. The method utilizes the unique focusing properties of azimuthally polarized phase vortex and radially polarized beam to independently excite a spinning(circularly polarized) magnetic dipole and linearly polarized dipole(perpendicular to the magnetic dipole) of a high index dielectric sphere.

  7. Plasma Limiter Based on Surface Wave Plasma Excited by Microwave

    Institute of Scientific and Technical Information of China (English)

    YANG Geng; TAN Jichun; SHEN Benjian

    2008-01-01

    A novel plasma limiter, in which the plasma is excited by surface wave, is presented. The breakdown time of some gases filled in the limiter were calculated as a function of gas pres-sure, ionization degree and density of seed electrons under low pressure (0.01 ~1 Torr) and high pressure (10 ~1000 Torr) cases. The results show that the limiter filled with Xe with a pressure of 0.9 Torr, seed electron density of 1016 m-3, and ionization degree of 10-4, has a breakdown time of approximate 19.6 ns.

  8. Giant Spin Pumping and Inverse Spin Hall Effect in the Presence of Surface and Bulk Spin-Orbit Coupling of Topological Insulator Bi2Se3.

    Science.gov (United States)

    Jamali, Mahdi; Lee, Joon Sue; Jeong, Jong Seok; Mahfouzi, Farzad; Lv, Yang; Zhao, Zhengyang; Nikolić, Branislav K; Mkhoyan, K Andre; Samarth, Nitin; Wang, Jian-Ping

    2015-10-14

    Three-dimensional (3D) topological insulators are known for their strong spin-orbit coupling (SOC) and the existence of spin-textured surface states that might be potentially exploited for "topological spintronics." Here, we use spin pumping and the inverse spin Hall effect to demonstrate successful spin injection at room temperature from a metallic ferromagnet (CoFeB) into the prototypical 3D topological insulator Bi2Se3. The spin pumping process, driven by the magnetization dynamics of the metallic ferromagnet, introduces a spin current into the topological insulator layer, resulting in a broadening of the ferromagnetic resonance (FMR) line width. Theoretical modeling of spin pumping through the surface of Bi2Se3, as well as of the measured angular dependence of spin-charge conversion signal, suggests that pumped spin current is first greatly enhanced by the surface SOC and then converted into a dc-voltage signal primarily by the inverse spin Hall effect due to SOC of the bulk of Bi2Se3. We find that the FMR line width broadens significantly (more than a factor of 5) and we deduce a spin Hall angle as large as 0.43 in the Bi2Se3 layer.

  9. Spin-transfer torque induced spin waves in antiferromagnetic insulators

    Science.gov (United States)

    Daniels, Matthew; Guo, Wei; Stocks, G. Malcolm; Xiao, Di; Xiao, Jiang

    2015-03-01

    We explore the possibility of exciting spin waves in insulating antiferromagnetic films by injecting spin current at the surface. We analyze both magnetically compensated and uncompensated interfaces. We find that the spin current induced spin-transfer torque can excite spin waves in insulating antiferromagnetic materials and that the chirality of the excited spin wave is determined by the polarization of the injected spin current. Furthermore, the presence of magnetic surface anisotropy can greatly increase the accessibility of these excitations. Supported by NSF EFRI-1433496 (M.W.D), U.S. DOE Office of Basic Energy Sciences, Materials Sciences and Engineering (D.X. & G.M.S.), Major State Basic Research Project of China and National Natural Science Foundation of China (W.G. and J.X.).

  10. Fractionalized spin-wave continuum in kagome spin liquids

    Science.gov (United States)

    Mei, Jia-Wei; Wen, Xiao-Gang

    Motivated by spin-wave continuum (SWC) observed in recent neutron scattering experiments in Herbertsmithite, we use Gutzwiller-projected wave functions to study dynamic spin structure factor S (q , ω) of spin liquid states on the kagome lattice. Spin-1 excited states in spin liquids are represented by Gutzwiller-projected two-spinon excited wave functions. We investigate three different spin liquid candidates, spinon Fermi-surface spin liquid (FSL), Dirac spin liquid (DSL) and random-flux spin liquid (RSL). FSL and RSL have low energy peaks in S (q , ω) at K points in the extended magnetic Brillouin zone, in contrast to experiments where low energy peaks are found at M points. There is no obviuos contradiction between DSL and neutron scattering measurements. Besides a fractionalized spin (i.e. spin-1/2), spinons in DSL carry a fractionalized crystal momentum which is potentially detectable in SWC in the neutron scattering measurements.

  11. Resonant Excitation of Terahertz Surface Plasmons in Subwavelength Metal Holes

    Directory of Open Access Journals (Sweden)

    Weili Zhang

    2007-01-01

    Full Text Available We present a review of experimental studies of resonant excitation of terahertz surface plasmons in two-dimensional arrays of subwavelength metal holes. Resonant transmission efficiency higher than unity was recently achieved when normalized to the area occupied by the holes. The effects of hole shape, hole dimensions, dielectric function of metals, polarization dependence, and array film thickness on resonant terahertz transmission in metal arrays were investigated by the state-of-the-art terahertz time-domain spectroscopy. In particular, extraordinary terahertz transmission was demonstrated in arrays of subwavelength holes made even from Pb, a generally poor metal, and having thickness of only one-third of skin depth. Terahertz surface plasmons have potential applications in terahertz imaging, biosensing, interconnects, and development of integrated plasmonic components for terahertz generation and detection.

  12. Quenching of magnetic excitations in single adsorbates at surfaces: Mn on CuN/Cu(100)

    Science.gov (United States)

    Novaes, Frederico D.; Lorente, Nicolás; Gauyacq, Jean-Pierre

    2010-10-01

    The lifetimes of spin excitations of Mn adsorbates on CuN/Cu(100) are computed from first principles. The theory is based on a strong-coupling approach that evaluates the decay of a spin excitation due to electron-hole pair creation. Using a previously developed theory [Phys. Rev. Lett. 103, 176601 (2009)10.1103/PhysRevLett.103.176601 and Phys. Rev. B 81, 165423 (2010)10.1103/PhysRevB.81.165423], we compute the excitation rates by a tunneling current for all the Mn spin states. A rate equation approach permits us to simulate the experimental results by Loth and co-workers [Nat. Phys. 6, 340 (2010)]10.1038/nphys1616 for large tunneling currents, taking into account the finite population of excited states. Our simulations give us insight into the spin dynamics, in particular, in the way polarized electrons can reveal the existence of an excited-state population. In addition, it reveals that the excitation process occurs in a way very different from the deexcitation one. Indeed, while excitation by tunneling electrons proceeds via the s and p electrons of the adsorbate, deexcitation mainly involves the d electrons.

  13. Parallel ferromagnetic resonance and spin-wave excitation in exchange-biased NiFe/IrMn bilayers

    Energy Technology Data Exchange (ETDEWEB)

    Sousa, Marcos Antonio de, E-mail: marcossharp@gmail.com [Instituto de Física, Universidade Federal de Goiás, Goiânia, 74001-970 (Brazil); Pelegrini, Fernando [Instituto de Física, Universidade Federal de Goiás, Goiânia, 74001-970 (Brazil); Alayo, Willian [Departamento de Física, Universidade Federal de Pelotas, Pelotas, 96010-900 (Brazil); Quispe-Marcatoma, Justiniano; Baggio-Saitovitch, Elisa [Centro Brasileiro de Pesquisas Físicas, Rio de Janeiro, 22290-180 (Brazil)

    2014-10-01

    Ferromagnetic Resonance study of sputtered Ru(7 nm)/NiFe(t{sub FM})/IrMn(6 nm)/Ru(5 nm) exchange-biased bilayers at X and Q-band microwave frequencies reveals the excitation of spin-wave and NiFe resonance modes. Angular variations of the in-plane resonance fields of spin-wave and NiFe resonance modes show the effect of the unidirectional anisotropy, which is about twice larger for the spin-wave mode due to spin pinning at the NiFe/IrMn interface. At Q-band frequency the angular variations of in-plane resonance fields also reveal the symmetry of a uniaxial anisotropy. A modified theoretical model which also includes the contribution of a rotatable anisotropy provides a good description of the experimental results.

  14. On the truncation of the number of excited states in density functional theory sum-over-states calculations of indirect spin spin coupling constants

    DEFF Research Database (Denmark)

    Zarycz, M. Natalia C.; Provasi, Patricio F.; Sauer, Stephan P. A.

    2015-01-01

    It is investigated, whether the number of excited (pseudo)states can be truncated in the sum-over-states expression for indirect spin-spin coupling constants (SSCC), which is used in the Contributions from Localized Orbitals within the Polarization Propagator Approach and Inner Projections......-correlation functional and the specialized core-property basis set, aug-cc-pVTZ-J. We investigated both how the calculated coupling constants depend on the number of (pseudo)states included in the summation and whether the summation can be truncated in a systematic way at a smaller number of states and extrapolated...... to the total number of (pseudo)states for the given one-electron basis set. We find that this is possible and that for some of the couplings it is sufficient to include only about 30% of the excited (pseudo)states....

  15. Mechanical back-action of a spin-wave resonance in a magnetoelastic thin film on a surface acoustic wave

    Science.gov (United States)

    Gowtham, P. G.; Labanowski, D.; Salahuddin, S.

    2016-07-01

    Surface acoustic waves (SAWs) traveling on the surface of a piezoelectric crystal can, through the magnetoelastic interaction, excite traveling spin-wave resonance in a magnetic film deposited on the substrate. This spin-wave resonance in the magnetic film creates a time-ynamic surface stress of magnetoelastic origin that acts back on the surface of the piezoelectric and modifies the SAW propagation. Unlike previous analyses that treat the excitation as a magnon-phonon polariton, here the magnetoelastic film is treated as a perturbation modifying boundary conditions on the SAW. We use acoustical perturbation theory to find closed-form expressions for the back-action surface stress and strain fields and the resultant SAW velocity shifts and attenuation. We demonstrate that the shear stres fields associated with this spin-wave back-action also generate effective surface currents on the piezoelectric both in phase and out of phase with the driving SAW potential. Characterization of these surface currents and their applications in determination of the magnetoelastic coupling are discussed. The perturbative calculation is carried out explicitly to first order (a regime corresponding to many experimental situations of current interest) and we provide a sketch of the implications of the theory at higher order.

  16. Molecular spin on surface: From strong correlation to dispersion interactions

    Science.gov (United States)

    Zhang, Yachao

    2016-09-01

    A reliable prediction of magnetic properties of surface-supported molecules containing 3d/4f spin carriers has challenged the electronic structure theory for decades. Here we tackle this problem with Hubbard-U corrected van der Waals density functional (vdW-DF), incorporating strong correlation effects of the localized electrons and dispersion interactions involved in the molecule-surface binding. By fitting the spin state energetics of a series of Fe(ii) compounds with varying ligand field strength, we find that the optimal U value for vdW-DF is much smaller than that for the local density approximation (LDA) while quite similar to that for the generalized gradient approximation (GGA). We show that although vdW-DF+U overestimates largely the metal-ligand bond distance, the predicted adiabatic high-spin-low-spin energy splitting ΔEHL is only slightly changed with respect to that obtained using the LDA+U geometries consistent with experiment. Then we use Cu(111)-supported metallocene (M(C5H5)2, M = Fe, and Co) as a prototype example to explore the effects of the molecule-surface interactions. We show that the non-local dispersion interactions, poorly described by LDA and GGA while reasonably captured by vdW-DF, are critical for reproducing ΔEHL at large molecule-surface distances. Besides, we find that ΔEHL is decreased by the molecule-metal contact, which is shown to weaken the local ligand field around the magnetic center.

  17. Ultrafast electron, lattice and spin dynamics on rare earth metal surfaces. Investigated with linear and nonlinear optical techniques

    Energy Technology Data Exchange (ETDEWEB)

    Radu, I.E.

    2006-03-15

    This thesis presents the femtosecond laser-induced electron, lattice and spin dynamics on two representative rare-earth systems: The ferromagnetic gadolinium Gd(0001) and the paramagnetic yttrium Y(0001) metals. The employed investigation tools are the time-resolved linear reflectivity and second-harmonic generation, which provide complementary information about the bulk and surface/interface dynamics, respectively. The femtosecond laser excitation of the exchange-split surface state of Gd(0001) triggers simultaneously the coherent vibrational dynamics of the lattice and spin subsystems in the surface region at a frequency of 3 THz. The coherent optical phonon corresponds to the vibration of the topmost atomic layer against the underlying bulk along the normal direction to the surface. The coupling mechanism between phonons and magnons is attributed to the modulation of the exchange interaction J between neighbour atoms due to the coherent lattice vibration. This leads to an oscillatory motion of the magnetic moments having the same frequency as the lattice vibration. Thus these results reveal a new type of phonon-magnon coupling mediated by the modulation of the exchange interaction and not by the conventional spin-orbit interaction. Moreover, we show that coherent spin dynamics in the THz frequency domain is achievable, which is at least one order of magnitude faster than previously reported. The laser-induced (de)magnetization dynamics of the ferromagnetic Gd(0001) thin films have been studied. Upon photo-excitation, the nonlinear magneto-optics measurements performed in this work show a sudden drop in the spin polarization of the surface state by more than 50% in a <100 fs time interval. Under comparable experimental conditions, the time-resolved photoemission studies reveal a constant exchange splitting of the surface state. The ultrafast decrease of spin polarization can be explained by the quasi-elastic spin-flip scattering of the hot electrons among spin

  18. The mutable nature of particle-core excitations with spin in the one-valence-proton nucleus 133Sb

    Directory of Open Access Journals (Sweden)

    G. Bocchi

    2016-09-01

    Full Text Available The γ-ray decay of excited states of the one-valence-proton nucleus 133Sb has been studied using cold-neutron induced fission of 235U and 241Pu targets, during the EXILL campaign at the ILL reactor in Grenoble. By using a highly efficient HPGe array, coincidences between γ-rays prompt with the fission event and those delayed up to several tens of microseconds were investigated, allowing to observe, for the first time, high-spin excited states above the 16.6 μs isomer. Lifetimes analysis, performed by fast-timing techniques with LaBr3(Ce scintillators, revealed a difference of almost two orders of magnitude in B(M1 strength for transitions between positive-parity medium-spin yrast states. The data are interpreted by a newly developed microscopic model which takes into account couplings between core excitations (both collective and non-collective of the doubly magic nucleus 132Sn and the valence proton, using the Skyrme effective interaction in a consistent way. The results point to a fast change in the nature of particle-core excitations with increasing spin.

  19. The mutable nature of particle-core excitations with spin in the one-valence-proton nucleus 133Sb

    Science.gov (United States)

    Bocchi, G.; Leoni, S.; Fornal, B.; Colò, G.; Bortignon, P. F.; Bottoni, S.; Bracco, A.; Michelagnoli, C.; Bazzacco, D.; Blanc, A.; de France, G.; Jentschel, M.; Köster, U.; Mutti, P.; Régis, J.-M.; Simpson, G.; Soldner, T.; Ur, C. A.; Urban, W.; Fraile, L. M.; Lozeva, R.; Belvito, B.; Benzoni, G.; Bruce, A.; Carroll, R.; Cieplicka-Oryǹczak, N.; Crespi, F. C. L.; Didierjean, F.; Jolie, J.; Korten, W.; Kröll, T.; Lalkovski, S.; Mach, H.; Mărginean, N.; Melon, B.; Mengoni, D.; Million, B.; Nannini, A.; Napoli, D.; Olaizola, B.; Paziy, V.; Podolyák, Zs.; Regan, P. H.; Saed-Samii, N.; Szpak, B.; Vedia, V.

    2016-09-01

    The γ-ray decay of excited states of the one-valence-proton nucleus 133Sb has been studied using cold-neutron induced fission of 235U and 241Pu targets, during the EXILL campaign at the ILL reactor in Grenoble. By using a highly efficient HPGe array, coincidences between γ-rays prompt with the fission event and those delayed up to several tens of microseconds were investigated, allowing to observe, for the first time, high-spin excited states above the 16.6 μs isomer. Lifetimes analysis, performed by fast-timing techniques with LaBr3(Ce) scintillators, revealed a difference of almost two orders of magnitude in B(M1) strength for transitions between positive-parity medium-spin yrast states. The data are interpreted by a newly developed microscopic model which takes into account couplings between core excitations (both collective and non-collective) of the doubly magic nucleus 132Sn and the valence proton, using the Skyrme effective interaction in a consistent way. The results point to a fast change in the nature of particle-core excitations with increasing spin.

  20. Effects of the spin-orbit and tensor interactions on the M1 and E2 excitations in light nuclei

    CERN Document Server

    Fayache, M S; Zamick, L; Von Neumann-Cosel, P; Richter, A

    1996-01-01

    The effects of varying the spin-orbit and tensor components of a realistic interaction on M1 excitation rates and B(E2)'s are studied on nuclei in the 0p and 1s-0d shells. Not only the total M1 but also the spin and orbital parts separately are studied. The single-particle energies are first calculated with the same interaction that is used between the valence nucleons. Later this stringent condition is relaxed somewhat and the 1s level is raised relative to 0d. For nuclei up to ^{28}Si, much better results i.e stronger B(M1) rates are obtained by increasing the strength of the spin-orbit interaction relative to the free value. This is probably also true for ^{32}S, but ^{36}Ar presents some difficulties. The effects of weakening the tensor interaction are also studied. On a more subtle level, the optimum spin-orbit interaction in the lower half of the s-d shell, as far as M1 excitations are concerned, is substantially larger than the difference E(J=3/2^+)_1-E(J=5/2^+)_1=5.2~MeV in ^{17}O. A larger spin-orbit...

  1. Cooling a mechanical resonator with nitrogen-vacancy centres using a room temperature excited state spin-strain interaction

    Science.gov (United States)

    Macquarrie, E. R.; Otten, M.; Gray, S. K.; Fuchs, G. D.

    2017-02-01

    Cooling a mechanical resonator mode to a sub-thermal state has been a long-standing challenge in physics. This pursuit has recently found traction in the field of optomechanics in which a mechanical mode is coupled to an optical cavity. An alternate method is to couple the resonator to a well-controlled two-level system. Here we propose a protocol to dissipatively cool a room temperature mechanical resonator using a nitrogen-vacancy centre ensemble. The spin ensemble is coupled to the resonator through its orbitally-averaged excited state, which has a spin-strain interaction that has not been previously studied. We experimentally demonstrate that the spin-strain coupling in the excited state is 13.5+/-0.5 times stronger than the ground state spin-strain coupling. We then theoretically show that this interaction, combined with a high-density spin ensemble, enables the cooling of a mechanical resonator from room temperature to a fraction of its thermal phonon occupancy.

  2. Disappearance of antiferromagnetic spin excitations in overdoped La2-xSrxCuO4.

    Science.gov (United States)

    Wakimoto, S; Yamada, K; Tranquada, J M; Frost, C D; Birgeneau, R J; Zhang, H

    2007-06-15

    Magnetic excitations for energies up to approximately 100 meV are studied for overdoped La(2-x)Sr(x)CuO(4) with x=0.25 and 0.30, using time-of-flight neutron spectroscopy. Comparison of spectra integrated over the width of an antiferromagnetic Brillouin zone demonstrates that the magnetic scattering at intermediate energies, 20 surface nesting, but rather is associated with a decreasing volume fraction of (probably fluctuating) antiferromagnetic bubbles.

  3. Measurement of Integrated Stokes Parameters for He 3 3p State Excited by Spin-Polarized Electrons

    Institute of Scientific and Technical Information of China (English)

    DING Hai-Bing; PANG Wen-Ning; LIU Yi-Bao; SHANG Ren-Cheng

    2005-01-01

    @@ Integrated Stokes parameters Pi (i = 1, 2, 3) for the He 3 3p → 2 3S1 (388.9nm) transition after excitation from the ground state to the 3 3 P state by a transversely spin-polarized electron beam are measured in near threshold energy region. The experimental results are presented. The linear-polarization P2 are consistent with zero over the incident energy range, providing evidence for the LS coupling mechanism of the 3 3P state. The measured circular polarization P3 are non-zero, indicating strong electron-electron exchange effects in the spin-polarized electron-atom collision process.

  4. Roles of Surface and Interface Spins in Exchange Coupled Nanostructures

    Science.gov (United States)

    Phan, Manh-Huong

    Exchange bias (EB) in magnetic nanostructures has remained a topic of global interest because of its potential use in spin valves, MRAM circuits, magnetic tunnel junctions, and spintronic devices. The exploration of EB on the nanoscale provides a novel approach to overcoming the superparamagnetic limit and increasing the thermoremanence of magnetic nanoparticles, a critical bottleneck for magnetic data storage applications. Recent advances in chemical synthesis have given us a unique opportunity to explore the EB in a variety of nanoparticle systems ranging from core/shell nanoparticles of Fe/γFe2O3, Co/CoO,and FeO/Fe3O4 to hollow nanoparticles of γFe2O3 and hybrid composite nanoparticles of Au/Fe3O4. Our studies have addressed the following fundamental and important questions: (i) Can one decouple collective contributions of the interface and surface spins to the EB in a core/shell nanoparticle system? (ii) Can the dynamic and static response of the core and shell be identified separately? (iii) Can one tune ``minor loop'' to ``exchange bias'' effects in magnetic hollow nanoparticles by varying the number of surface spins? (iv) Can one decouple collective contributions of the inner and outer surface spins to the EB in a hollow nanoparticle system? (v) Can EB be induced in a magnetic nanoparticle by forming its interface with a non-magnetic metal? Such knowledge is essential to tailor EB in magnetic nanostructures for spintronics applications. In this talk, we will discuss the aforementioned findings in terms of our experimental and atomistic Monte Carlo studies. The work was supported by the U.S. Department of Energy, Office of Basic Energy Sciences, Division of Materials Sciences and Engineering under Award No. DE-FG02-07ER46438.

  5. Nuclear response theory for spin-isospin excitations in a relativistic quasiparticle-phonon coupling framework

    Science.gov (United States)

    Robin, Caroline; Litvinova, Elena

    2016-07-01

    A new theoretical approach to spin-isospin excitations in open-shell nuclei is presented. The developed method is based on the relativistic meson-exchange nuclear Lagrangian of Quantum Hadrodynamics and extends the response theory for superfluid nuclear systems beyond relativistic quasiparticle random phase approximation in the proton-neutron channel (pn-RQRPA). The coupling between quasiparticle degrees of freedom and collective vibrations (phonons) introduces a time-dependent effective interaction, in addition to the exchange of pion and ρ -meson taken into account without retardation. The time-dependent contributions are treated in the resonant time-blocking approximation, in analogy to the previously developed relativistic quasiparticle time-blocking approximation (RQTBA) in the neutral (non-isospin-flip) channel. The new method is called proton-neutron RQTBA (pn-RQTBA) and is applied to the Gamow-Teller resonance in a chain of neutron-rich nickel isotopes 68-78Ni . A strong fragmentation of the resonance along with quenching of the strength, as compared to pn-RQRPA, is obtained. Based on the calculated strength distribution, beta-decay half-lives of the considered isotopes are computed and compared to pn-RQRPA half-lives and to experimental data. It is shown that a considerable improvement of the half-life description is obtained in pn-RQTBA because of the spreading effects, which bring the lifetimes to a very good quantitative agreement with data.

  6. Surface-enhanced Raman scattering on aluminum using near infrared and visible excitation

    DEFF Research Database (Denmark)

    Mogensen, Klaus Bo; Gühlke, Marina; Kneipp, Janina;

    2014-01-01

    We observed strong surface-enhanced Raman scattering on discontinuous nanostructured aluminum films using 785 nm excitation even though dielectric constants of this metal suggest plasmon supported spectroscopy in the ultraviolet range. The excitation of SERS correlates with plasmon resonances...

  7. Intrinsic spin dynamics in optically excited nanoscale magnetic tunnel junction arrays restored by dielectric coating

    Science.gov (United States)

    Jaris, M.; Yahagi, Y.; Mahato, B. K.; Dhuey, S.; Cabrini, S.; Nikitin, V.; Stout, J.; Hawkins, A. R.; Schmidt, H.

    2016-11-01

    We report the all-optical observation of intrinsic spin dynamics and extraction of magnetic material parameters from arrays of sub-100 nm spin-transfer torque magnetic random access memory (STT-MRAM) devices with a CoFeB/MgO interface. To this end, the interference of surface acoustic waves with time-resolved magneto-optic signals via magneto-elastic coupling was suppressed using a dielectric coating. The efficacy of this method is demonstrated experimentally and via modeling on a nickel nanomagnet array. The magnetization dynamics for both coated nickel and STT-MRAM arrays shows a restored field-dependent Kittel mode from which the effective damping can be extracted. We observe an increased low-field damping due to extrinsic contributions from magnetic inhomogeneities and variations in the nanomagnet shape, while the intrinsic Gilbert damping remains unaffected by patterning. The data are in excellent agreement with a local resonance model and have direct implications for the design of STT-MRAM devices as well as other nanoscale spintronic technologies.

  8. High-spin states of 125Sb: Particle-core excitation coupling

    Institute of Scientific and Technical Information of China (English)

    LIU; Zhong; (

    2003-01-01

    [1]Fogelberg, B., Carle, P., Levels and transition probabilities in 120,122,124,126,128Sn studied in the decay of In isotopes, Nucl. Phys. A, 1979, 323: 205-252.[2]Broda, R., Mayer, R. H., Bearden, I. G. et al., Yrast isomers in tin nuclei from heavy ion collisions and the νh11/2 subshell filling, Phys. Rev. Lett., 1992, 68: 1671-1674.[3]Stone, C. A., Walters, W. B., Decay of 17-min (19/2)- 129mSb, Z. Phys. A, 1987, 328: 257-258.[4]Genevey, J., Pinston, J. A., Faust, H., New high-spin microsecond isomers in 131Sb, Eur. Phys. J., 2000, A9: 191-195.[5]Shroy, R. E., Gaigalas, A. K., Schatz, G. et al., High-spin states in odd-mass 113-119Sb: △J = 1 bands on 9/2+ proton-hole states, Phys. Rev. C, 1979, 19: 1324-1343.[6]Lunardi, S., Daly, P. J., Soramel, F. et al., Decay of (Vh11/2n)10+ and (πd5/2Vh11/2n)25/2+ isomers in even-A Sn and odd-A Sb nuclei, Z. Phys. A, 1987, 328: 487-492.[7]Piel, W. F. Jr., Chowdhury, P., Garg, U. et al., Collective structures in the odd-Z transitional nuclei 115,117I and 121,123Sb, Phys. Rev. C, 1985, 31: 456-464.[8]Katakura, J., Nuclear data sheets for A = 125. Nuclear Data Sheets, 1999, 86: 981-990.[9]Morinaga, H., Yamazaki, T., In-beam Gamma-ray Spectroscopy, Amsterdam: North-Holland Publishing Company, 1976, 324-332.[10]Zhang, C. T., Bhattacharyya, P., Daly, P. J. et al., Yrast excitations in A = 126-131 Te nuclei from deep inelastic 130Te + 64Ni reactions, Nucl. Phys. A, 1998, 628: 386-402.[11]Apt, K. E., Walters, W. B., Radioactive decay of 2.2-h 127Sn to levels of 127Sb, Phys. Rev. C, 1974, 9: 310-325.[12]Jonsson, N. -G., Backlin, A., Kantele, J. et al., Collective states in even Sn nuclei, Nucl. Phys. A, 1981, 371: 333-348.[13]Vanden, G., Berghe, H. K., Structure and electromagnetic properties of the odd-A antimony isotopes in a unified-model calculation, Nucl. Phys. A,1971, 163: 478-512.[14]Blomqvist, J., Kleinheinz, P., Daly, P. J., Atomic masses above 146Gd derived from a

  9. Entanglement and localization of the one spin excitation states in a quantum $XX$ chain with a impurity

    CERN Document Server

    Zwick, A

    2009-01-01

    One spin excitation states are involved in the transmission of quantum states and entanglement through a quantum spin chain, the localization properties of these states are crucial to achieve the transfer of information from one extreme of the chain to the other. We investigate the bipartite entanglement and localization of the one excitation states in a quantum $XX$ chain with one impurity. The bipartite entanglement is obtained using the Concurrence and the localization is analyzed using the inverse participation ratio. Changing the strength of the exchange coupling of the impurity allows us to control the number of localized or extended states. Our results show that equally localized states do not possess the same bipartite entanglement and suggest that only a restricted class of localizated states allows the storage and transmission of quantum states.

  10. Quantum Entanglement Channel based on Excited States in a Spin Chain

    Institute of Scientific and Technical Information of China (English)

    张少良; 杜良辉; 郭光灿; 周幸祥; 周正威

    2011-01-01

    We study the possibility of using a spin chain to construct a quantum entanglement channel that can be used for quantum state transmission in a solid state system.We analyze the spin chain's states under various z-directional magnetic field and spin interactions to determine the entanglement between Alice and Bob's spins.We derive the conditions under which this entanglement can be distilled,and find that a spin chain of arbitrary length can be used as a quantum channel for quantum state transmission when the number of spin flips in the chain is large.%We study the possibility of using a spin chain to construct a quantum entanglement channel that can be used for quantum state transmission in a solid state system. We analyze the spin chain's states under various z-directional magnetic field and spin interactions to determine the entanglement between Alice and Bob's spins. We derive the conditions under which this entanglement can be distilled, and find that a spin chain of arbitrary length can be used as a quantum channel for quantum state transmission when the number of spin Hips in the chain is large.

  11. Interference of spin states in photoemission from Sb/Ag(111) surface alloys

    Energy Technology Data Exchange (ETDEWEB)

    Meier, Fabian; Osterwalder, Juerg; Hugo Dil, J [Physik-Institut, Universitaet Zuerich, Winterthurerstrasse 190, CH-8057 Zuerich (Switzerland); Petrov, Vladimir [St Petersburg Polytechnical University, 29 Polytechnicheskaya Street, 195251 St Petersburg (Russian Federation); Mirhosseini, Hossein; Henk, Juergen [Max-Planck-Institut fuer Mikrostrukturphysik, D-06120 Halle (Saale) (Germany); Patthey, Luc, E-mail: jan-hugo.dil@psi.ch [Swiss Light Source, Paul Scherrer Institut, CH-5232 Villigen (Switzerland)

    2011-02-23

    Using a three-dimensional spin polarimeter we have gathered evidence for the interference of spin states in photoemission from the surface alloy Sb/Ag(111). This system features a small Rashba-type spin splitting of a size comparable to the momentum broadening of the quasiparticles, thus causing an intrinsic overlap between states with orthogonal spinors. Besides a small spin polarization caused by the spin splitting, we observe a large spin polarization component in the plane normal to the quantization axis of the Rashba effect. Strongly suggestive of coherent spin rotation, this effect is largely independent of the photon energy and photon polarization. (fast track communication)

  12. Excitation and tailoring of diffractive spin-wave beams in NiFe using nonuniform microwave antennas

    Science.gov (United States)

    Körner, H. S.; Stigloher, J.; Back, C. H.

    2017-09-01

    We experimentally demonstrate by time-resolved scanning magneto-optical Kerr microscopy the possibility to locally excite multiple spin-wave beams in the dipolar-dominated regime in metallic NiFe films. For this purpose we employ differently shaped nonuniform microwave antennas consisting of several coplanar waveguide sections different in size, thereby adapting an approach for the generation of spin-wave beams in the exchange-dominated regime suggested by Gruszecki et al. [Sci. Rep. 6, 22367 (2016), 10.1038/srep22367]. The occurring spin-wave beams are diffractive and we show that the width of the beam and its widening as it propagates can be tailored by the shape and the length of the nonuniformity. Moreover, the propagation direction of the diffractive beams can be manipulated by changing the bias field direction.

  13. Spin fluctuations and excitations in a 2D xy-ferromagnet: CoCl/sub 2/ in graphite

    Energy Technology Data Exchange (ETDEWEB)

    Wiesler, D.G.; Zabel, H.

    1989-01-01

    We have investigated by neutron scattering the spin fluctuations and excitations in the stage 2 CoCl/sub 2/ -- graphite intercalation compound. This compound has easy-plane anisotropy and sufficiently weak interplanar interaction to qualify as a test material for Kosterlitz-Thouless-Berezinsky type phase transitions. We have carried out quasi-elastic scattering measurements to determine the temperature variation of the spin correlation length /xi/ above the two dimensional ordering transition. We have also probed the dependence on wave vector and temperature of the inelastic scattering cross section, consisting of both a central peak, associated with vortex diffusion, and spin wave, which become strongly damped above the transition temperature. 15 refs., 5 figs.

  14. Spin wave absorber generated by artificial surface anisotropy for spin wave device network

    Science.gov (United States)

    Kanazawa, Naoki; Goto, Taichi; Sekiguchi, Koji; Granovsky, Alexander B.; Takagi, Hiroyuki; Nakamura, Yuichi; Inoue, Mitsuteru

    2016-09-01

    Spin waves (SWs) have the potential to reduce the electric energy loss in signal processing networks. The SWs called magnetostatic forward volume waves (MSFVWs) are advantageous for networking due to their isotropic dispersion in the plane of a device. To control the MSFVW flow in a processing network based on yttrium iron garnet, we developed a SW absorber using artificial structures. The mechanical surface polishing method presented in this work can well control extrinsic damping without changing the SW dispersion of the host material. Furthermore, enhancement of the ferromagnetic resonance linewidth over 3 Oe was demonstrated.

  15. On the truncation of the number of excited states in density functional theory sum-over-states calculations of indirect spin spin coupling constants

    Energy Technology Data Exchange (ETDEWEB)

    Zarycz, M. Natalia C., E-mail: mnzarycz@gmail.com; Provasi, Patricio F., E-mail: patricio@unne.edu.ar [Department of Physics, University of Northeastern - CONICET, Av. Libertad 5500, Corrientes W3404AAS (Argentina); Sauer, Stephan P. A., E-mail: sauer@kiku.dk [Department of Chemistry, University of Copenhagen, Universitetsparken 5, DK-2100 Copenhagen Ø (Denmark)

    2015-12-28

    It is investigated, whether the number of excited (pseudo)states can be truncated in the sum-over-states expression for indirect spin-spin coupling constants (SSCCs), which is used in the Contributions from Localized Orbitals within the Polarization Propagator Approach and Inner Projections of the Polarization Propagator (IPPP-CLOPPA) approach to analyzing SSCCs in terms of localized orbitals. As a test set we have studied the nine simple compounds, CH{sub 4}, NH{sub 3}, H{sub 2}O, SiH{sub 4}, PH{sub 3}, SH{sub 2}, C{sub 2}H{sub 2}, C{sub 2}H{sub 4}, and C{sub 2}H{sub 6}. The excited (pseudo)states were obtained from time-dependent density functional theory (TD-DFT) calculations with the B3LYP exchange-correlation functional and the specialized core-property basis set, aug-cc-pVTZ-J. We investigated both how the calculated coupling constants depend on the number of (pseudo)states included in the summation and whether the summation can be truncated in a systematic way at a smaller number of states and extrapolated to the total number of (pseudo)states for the given one-electron basis set. We find that this is possible and that for some of the couplings it is sufficient to include only about 30% of the excited (pseudo)states.

  16. On the truncation of the number of excited states in density functional theory sum-over-states calculations of indirect spin spin coupling constants.

    Science.gov (United States)

    Zarycz, M Natalia C; Provasi, Patricio F; Sauer, Stephan P A

    2015-12-28

    It is investigated, whether the number of excited (pseudo)states can be truncated in the sum-over-states expression for indirect spin-spin coupling constants (SSCCs), which is used in the Contributions from Localized Orbitals within the Polarization Propagator Approach and Inner Projections of the Polarization Propagator (IPPP-CLOPPA) approach to analyzing SSCCs in terms of localized orbitals. As a test set we have studied the nine simple compounds, CH4, NH3, H2O, SiH4, PH3, SH2, C2H2, C2H4, and C2H6. The excited (pseudo)states were obtained from time-dependent density functional theory (TD-DFT) calculations with the B3LYP exchange-correlation functional and the specialized core-property basis set, aug-cc-pVTZ-J. We investigated both how the calculated coupling constants depend on the number of (pseudo)states included in the summation and whether the summation can be truncated in a systematic way at a smaller number of states and extrapolated to the total number of (pseudo)states for the given one-electron basis set. We find that this is possible and that for some of the couplings it is sufficient to include only about 30% of the excited (pseudo)states.

  17. Rashba-type spin splitting and spin interference of the Cu(1 1 1) surface state at room temperature

    Energy Technology Data Exchange (ETDEWEB)

    Dil, J. Hugo, E-mail: hugo.dil@epfl.ch [Institut de Physique de la Matière Condensée, Ecole Polytechnique Fédérale de Lausanne, CH-1015 Lausanne (Switzerland); Physik-Institut, Universität Zürich, Winterthurerstrasse 190, CH-8057 Zürich (Switzerland); Swiss Light Source, Paul Scherrer Institut, CH-5232 Villigen (Switzerland); Meier, Fabian [Physik-Institut, Universität Zürich, Winterthurerstrasse 190, CH-8057 Zürich (Switzerland); Swiss Light Source, Paul Scherrer Institut, CH-5232 Villigen (Switzerland); Osterwalder, Jürg [Physik-Institut, Universität Zürich, Winterthurerstrasse 190, CH-8057 Zürich (Switzerland)

    2015-05-15

    We report on the measurement of the Rashba-type spin splitting of the Shockley surface state on Cu(1 1 1) by spin- and angle-resolved photoemission at room temperature. Along the spatial direction expected for a Rashba-type effect the measured spin splitting corresponds to what has previously been reported by first principle calculations which were verified by high resolution ARPES using low temperatures and perfect crystals. Furthermore it is found that structural defects cause a spin-interference in the photoemission process and as a result the main measured spin signal is in the plane orthogonal to the typical Rashba orientation. Although the determination of the exact origin of this signal requires further investigations, the main results can be used as a benchmark for future spin-resolved photoemission set-ups.

  18. Spin density wave order, topological order, and Fermi surface reconstruction

    CERN Document Server

    Sachdev, Subir; Chatterjee, Shubhayu; Schattner, Yoni

    2016-01-01

    In the conventional theory of density wave ordering in metals, the onset of spin density wave (SDW) order co-incides with the reconstruction of the Fermi surfaces into small 'pockets'. We present models which display this transition, while also displaying an alternative route between these phases via an intermediate phase with topological order, no broken symmetry, and pocket Fermi surfaces. The models involve coupling emergent gauge fields to a fractionalized SDW order, but retain the canonical electron operator in the underlying Hamiltonian. We establish an intimate connection between the suppression of certain defects in the SDW order, and the presence of Fermi surface sizes distinct from the Luttinger value in Fermi liquids. We discuss the relevance of such models to the physics of the hole-doped cuprates near optimal doping.

  19. Fermi surface versus Fermi sea contributions to intrinsic anomalous and spin Hall effects of multiorbital metals in the presence of Coulomb interaction and spin-Coulomb drag

    Science.gov (United States)

    Arakawa, Naoya

    2016-06-01

    Anomalous Hall effect (AHE) and spin Hall effect (SHE) are fundamental phenomena, and their potential for application is great. However, we understand the interaction effects unsatisfactorily, and should have clarified issues about the roles of the Fermi sea term and Fermi surface term of the conductivity of the intrinsic AHE or SHE of an interacting multiorbital metal and about the effects of spin-Coulomb drag on the intrinsic SHE. Here, we resolve the first issue and provide the first step about the second issue by developing a general formalism in the linear response theory with appropriate approximations and using analytic arguments. The most striking result is that even without impurities, the Fermi surface term, a non-Berry-curvature term, plays dominant roles at high or slightly low temperatures. In particular, this Fermi surface term causes the temperature dependence of the dc anomalous Hall or spin Hall conductivity due to the interaction-induced quasiparticle damping and the correction of the dc spin Hall conductivity due to the spin-Coulomb drag. Those results revise our understanding of the intrinsic AHE and SHE. We also find that the differences between the dc anomalous Hall and longitudinal conductivities arise from the difference in the dominant multiband excitations. This not only explains why the Fermi sea term such as the Berry-curvature term becomes important in clean and low-temperature case only for interband transports, but also provides the useful principles on treating the electron-electron interaction in an interacting multiorbital metal for general formalism of transport coefficients. Several correspondences between our results and experiments are finally discussed.

  20. Solid-State Selective 13C Excitation and Spin Diffusion NMR to Resolve Spatial Dimensions in Plant Cell Walls

    Energy Technology Data Exchange (ETDEWEB)

    Foston, M.; Katahira, R.; Gjersing, E.; Davis, M. F.; Ragauskas, A. J.

    2012-02-15

    The average spatial dimensions between major biopolymers within the plant cell wall can be resolved using a solid-state NMR technique referred to as a {sup 13}C cross-polarization (CP) SELDOM (selectively by destruction of magnetization) with a mixing time delay for spin diffusion. Selective excitation of specific aromatic lignin carbons indicates that lignin is in close proximity to hemicellulose followed by amorphous and finally crystalline cellulose. {sup 13}C spin diffusion time constants (T{sub SD}) were extracted using a two-site spin diffusion theory developed for {sup 13}C nuclei under magic angle spinning (MAS) conditions. These time constants were then used to calculate an average lower-limit spin diffusion length between chemical groups within the plant cell wall. The results on untreated {sup 13}C enriched corn stover stem reveal that the lignin carbons are, on average, located at distances {approx}0.7-2.0 nm from the carbons in hemicellulose and cellulose, whereas the pretreated material had larger separations.

  1. Excited state potential energy surfaces and their interactions in Fe(IV)=O active sites.

    Science.gov (United States)

    Srnec, Martin; Wong, Shaun D; Solomon, Edward I

    2014-12-21

    The non-heme ferryl active sites are of significant interest for their application in biomedical and green catalysis. These sites have been shown to have an S = 1 or S = 2 ground spin state; the latter is functional in biology. Low-temperature magnetic circular dichroism (LT MCD) spectroscopy probes the nature of the excited states in these species including ligand-field (LF) states that are otherwise difficult to study by other spectroscopies. In particular, the temperature dependences of MCD features enable their unambiguous assignment and thus determination of the low-lying excited states in two prototypical S = 1 and S = 2 NHFe(IV)[double bond, length as m-dash]O complexes. Furthermore, some MCD bands exhibit vibronic structures that allow mapping of excited-state interactions and their effects on the potential energy surfaces (PESs). For the S = 2 species, there is also an unusual spectral feature in both near-infrared absorption and MCD spectra - Fano antiresonance (dip in Abs) and Fano resonance (sharp peak in MCD) that indicates the weak spin-orbit coupling of an S = 1 state with the S = 2 LF state. These experimental data are correlated with quantum-chemical calculations that are further extended to analyze the low-lying electronic states and the evolution of their multiconfigurational characters along the Fe-O PESs. These investigations show that the lowest-energy states develop oxyl Fe(III) character at distances that are relevant to the transition state (TS) for H-atom abstraction and define the frontier molecular orbitals that participate in the reactivity of S = 1 vs. S = 2 non-heme Fe(IV)[double bond, length as m-dash]O active sites. The S = 1 species has only one available channel that requires the C-H bond of a substrate to approach perpendicular to the Fe-oxo bond (the π channel). In contrast, there are three channels (one σ and two π) available for the S = 2 non-heme Fe(IV)[double bond, length as m-dash]O system allowing C-H substrate approach

  2. Two Dimensional Incommensurate Spin Excitations and Lattice Fluctuations in La2 - x Bax CuO4

    Science.gov (United States)

    Wagman, J. J.; Carlo, J. P.; van Gastel, G.; Zhao, Y.; Kallin, A. B.; Mazurek, E.; Dabkowska, H. A.; Savicii, A.; Granroth, G. E.; Yamani, Z.; Tun, Z.; Gaulin, B. D.

    2013-03-01

    'Hour-glass' shaped dispersions of antiferromagnetic (AF) spin fluctuations are a robust feature common to many high temperature superconductors. In 214 cuprates, these phenomena are well known to display a strong dependence on the concentration of holes that are introduced into the copper oxide planes by doping. The incommensurability (IC) of the two dimensional magnetic order in this system is sensitive to hole concentration. Here, we present a series of neutron scattering measurements on single crystals of La2 - x Bax CuO4 (LBCO), with 0 . 035 <= x <= 0 . 095 , a doping range that spans the transition from diagonal to parallel IC ordering wavevectors, and from non-superconducting to superconducting ground states. Our measurements map out the evolution of the spin excitations for energies below ~ 50 meV, and focus on an enhancement in the scattered intensity centered in the 17-20 meV at the AF IC positions. This regime corresponds to the approximate crossing of very dispersive spin excitations and weakly dispersive low lying optic phonons in LBCO. NSERC, Scientific User Facilities Division, Office of Basic Energy Sciences, U.S. Department of Energy

  3. Ultrafast x-ray diffraction thermometry measures the influence of spin excitations on the heat transport through nanolayers

    Science.gov (United States)

    Koc, A.; Reinhardt, M.; von Reppert, A.; Rössle, M.; Leitenberger, W.; Dumesnil, K.; Gaal, P.; Zamponi, F.; Bargheer, M.

    2017-07-01

    We investigate the heat transport through a rare earth multilayer system composed of yttrium (Y), dysprosium (Dy), and niobium (Nb) by ultrafast x-ray diffraction. This is an example of a complex heat flow problem on the nanoscale, where several different quasiparticles carry the heat and conserve a nonequilibrium for more than 10 ns. The Bragg peak positions of each layer represent layer-specific thermometers that measure the energy flow through the sample after excitation of the Y top layer with fs-laser pulses. In an experiment-based analytic solution to the nonequilibrium heat transport problem, we derive the individual contributions of the spins and the coupled electron-lattice system to the heat conduction. The full characterization of the spatiotemporal energy flow at different starting temperatures reveals that the spin excitations of antiferromagnetic Dy speed up the heat transport into the Dy layer at low temperatures, whereas the heat transport through this layer and further into the Y and Nb layers underneath is slowed down. The experimental findings are compared to the solution of the heat equation using macroscopic temperature-dependent material parameters without separation of spin and phonon contributions to the heat. We explain why the simulated energy density matches our experiment-based derivation of the heat transport, although the simulated thermoelastic strain in this simulation is not even in qualitative agreement.

  4. Cotunneling spectroscopy and the properties of excited-state spin manifolds of Mn12 single molecule magnets

    Science.gov (United States)

    Rostamzadeh Renani, Fatemeh; Kirczenow, George

    2014-10-01

    We study charge transport through single molecule magnet (SMM) junctions in the cotunneling regime as a tool for investigating the properties of the excited-state manifolds of neutral Mn12 SMs. This study is motivated by a recent transport experiment [S. Kahle et al., Nano Lett. 12, 518 (2012), 10.1021/nl204141z] that probed the details of the magnetic and electronic structure of Mn12 SMMs beyond the ground-state spin manifold. A giant spin Hamiltonian and master equation approach is used to explore theoretically the cotunneling transport through Mn12-Ac SMM junctions. We identify SMM transitions that can account for both the strong and weak features of the experimental differential conductance spectra. We find the experimental results to imply that the excited spin-state manifolds of the neutral SMM have either different anisotropy constants or different g factors in comparison with its ground-state manifold. However, the latter scenario accounts best for the experimental data.

  5. Spin Canting and Transverse Relaxation at Surfaces and in the Interior of Ferrimagnetic Particles

    DEFF Research Database (Denmark)

    Mørup, Steen

    2003-01-01

    Analytical expressions for the magnetic energy and the spin-canting angles in some simple ferrimagnetic bulk and surface structures are presented. It is shown that the energy barriers separating different spin-canted states often will be very small. Therefore, the spin canting may be static only ...

  6. The mutable nature of particle-core excitations with spin in the one-valence-proton nucleus 133Sb

    CERN Document Server

    Bocchi, G; Fornal, B; Colo', G; Bortignon, P F; Bottoni, S; Bracco, A; Michelagnoli, C; Bazzacco, D; Blanc, A; De France, G; Jentschel, M; Koster, U; Mutti, P; Regis, J -M; Simpson, G; Soldner, T; Ur, C A; Urban, W; Fraile, L M; Lozeva, R; Belvito, B; Benzoni, G; Bruce, A; Carroll, R; Cieplicka-Orynczak, N; Crespi, F C L; Didierjean, F; Jolie, J; Korten, W; Kroll, T; Lalkovski, S; Mach, H; Marginean, N; Melon, B; Mengoni, D; Million, B; Nannini, A; Napoli, D; Olaizola, B; Paziy, V; Podolyakn, Zs; Regann, P H; Saed-Samii, N; Szpak, B; Vedia, V

    2016-01-01

    The gamma-ray decay of excited states of the one-valence-proton nucleus 133Sb has been studied using cold-neutron induced fission of 235U and 241Pu targets, during the EXILL campaign at the ILL reactor in Grenoble. By using a highly efficient HPGe array, coincidences between gamma-rays prompt with the fission event and those delayed up to several tens of microseconds were investigated, allowing to observe, for the first time, high-spin excited states above the 16.6 micros isomer. Lifetimes analysis, performed by fast-timing techniques with LaBr3(Ce) scintillators, reveals a difference of almost two orders of magnitude in B(M1) strength for transitions between positive-parity medium-spin yrast states. The data are interpreted by a newly developed microscopic model which takes into account couplings between core excitations (both collective and non-collective) of the doubly magic nucleus 132Sn and the valence proton, using the Skyrme effective interaction in a consistent way. The results point to a fast change ...

  7. Functionally graded piezoelectric materials for modal transducers for exciting bulk and surface acoustic waves.

    Science.gov (United States)

    Yang, Jiashi; Jin, Zhihe; Li, Jiangyu

    2008-07-01

    We show that functionally graded piezoelectric materials can be used to make modal actuators through theoretical analyses of the excitation of extensional motion in an elastic rod and Rayleigh surface waves over an elastic half-plane. The results suggest alternatives with certain advantages for the excitation of bulk and surface acoustic waves.

  8. Compact surface structures for the efficient excitation of surface plasmon-polaritons

    Energy Technology Data Exchange (ETDEWEB)

    De la Cruz, S.; Mendez, E.R. [Division de Fisica Applicada, Centro de Investigacion Cientifica y de Educacion Superior de Ensenada, Carretera Ensenada-Tijuana No. 3918, Ensenada 22860, BC (Mexico); Macias, D.; Salas-Montiel, R.; Adam, P.M. [Laboratoire de Nanotechnologie et d' Instrumentation Optique, Universite de Technologie de Troyes, 12 rue Marie Curie, BP-2060, 10010 Troyes Cedex (France)

    2012-06-15

    We present calculations of the efficiency of excitation of surface plasmon-polaritons (SPPs) with surface structures illuminated by focussed beams. First, it is shown that the low reflectivity observed with broad highly directional beams and periodic gratings does not necessarily imply an efficient coupling to SPPs. We then consider the coupling through surface features like steps, grooves and angled steps, and calculate efficiency maps for these structures as functions of the parameters that define them. Finally, we explore the possibilities of improving the coupling efficiency using periodic structures consisting of a small number of rectangular grooves. We find that a surface section with a length of about four wavelengths can couple as much as 45% of the incident light into a directional SPP. (Copyright copyright 2012 WILEY-VCH Verlag GmbH and Co. KGaA, Weinheim)

  9. Non-orthogonal spin-adaptation of coupled cluster methods: A new implementation of methods including quadruple excitations

    Science.gov (United States)

    Matthews, Devin A.; Stanton, John F.

    2015-02-01

    The theory of non-orthogonal spin-adaptation for closed-shell molecular systems is applied to coupled cluster methods with quadruple excitations (CCSDTQ). Calculations at this level of detail are of critical importance in describing the properties of molecular systems to an accuracy which can meet or exceed modern experimental techniques. Such calculations are of significant (and growing) importance in such fields as thermodynamics, kinetics, and atomic and molecular spectroscopies. With respect to the implementation of CCSDTQ and related methods, we show that there are significant advantages to non-orthogonal spin-adaption with respect to simplification and factorization of the working equations and to creating an efficient implementation. The resulting algorithm is implemented in the CFOUR program suite for CCSDT, CCSDTQ, and various approximate methods (CCSD(T), CC3, CCSDT-n, and CCSDT(Q)).

  10. A Green's function model for ferromagnetism and spin excitations of (Ga, Mn)As diluted magnetic semiconductors

    Institute of Scientific and Technical Information of China (English)

    Liu Gui-Bin; Liu Bang-Gui

    2009-01-01

    We study (Ga, Mn)As diluted magnetic semiconductors in terms of the Ruderman-Kittel-Kasuya-Yosida quantum spin model in Green's function approach. Random distributions of the magnetic atoms are treated by using an analytical average of magnetic configurations. Average magnetic moments and spin excitation spectra as functions of temperature can be obtained by solving self-consistent equations, and the Curie temperature T_C is given explicitly. T_C is proportional to magnetic atomic concentration, and there exists a maximum for T_C as a function of carrier concentration. Applied to (Ga, Mn)As, the theoretical results are consistent with experiment and the experimental T_C can be obtained with reasonable parameters. This modelling can also be applied to other diluted magnetic semiconductors.

  11. Delta self-consistent field method to obtain potential energy surfaces of excited molecules on surfaces

    DEFF Research Database (Denmark)

    Gavnholt, Jeppe; Olsen, Thomas; Engelund, Mads;

    2008-01-01

    We present a modification of the Delta self-consistent field (Delta SCF) method of calculating energies of excited states in order to make it applicable to resonance calculations of molecules adsorbed on metal surfaces, where the molecular orbitals are highly hybridized. The Delta SCF approximation...... is a density-functional method closely resembling standard density-functional theory (DFT), the only difference being that in Delta SCF one or more electrons are placed in higher lying Kohn-Sham orbitals instead of placing all electrons in the lowest possible orbitals as one does when calculating the ground......-state energy within standard DFT. We extend the Delta SCF method by allowing excited electrons to occupy orbitals which are linear combinations of Kohn-Sham orbitals. With this extra freedom it is possible to place charge locally on adsorbed molecules in the calculations, such that resonance energies can...

  12. Surface spin disorder and spin-glass-like behaviour in manganese-substituted cobalt ferrite nanoparticles

    Science.gov (United States)

    Topkaya, R.; Akman, Ö.; Kazan, S.; Aktaş, B.; Durmus, Z.; Baykal, A.

    2012-10-01

    Manganese-substituted cobalt ferrite nanoparticles coated with triethylene glycol (TREG) have been prepared by the glycothermal reaction. The effect of Mn substitution and coating on temperature-dependent magnetic properties of the TREG-coated Mn x Co1- x Fe2O4 nanoparticles (0.0 ≤ x ≤ 0.8) with size of 5-7 nm has been investigated in the temperature range of 10-300 K in a magnetic field up to 9 T. After the irreversible processes of the magnetic hysteresis curves were completed, the high-field regions of these curves were fitted by using a `law of approach to saturation' to extract the magnetic properties, such as the effective anisotropy constant ( K eff) and the anisotropy field ( H A) etc. High coercive field of 12.6 kOe is observed in pure cobalt ferrite coated with TREG at 10 K. The low temperature unsaturated magnetization behaviour indicates the core-shell structure of the Mn x Co1- x Fe2O4 NPs. Zero-field-cooled (ZFC) and field-cooled (FC) measurements revealed superparamagnetic phase of TREG-coated Mn x Co1- x Fe2O4 nanoparticles at room temperature. The blocking and irreversibility temperatures obtained from ZFC-FC curves decrease at highest Mn concentration ( x = 0.8). The existence of spin-glass-like surface layer with freezing temperature of 215 K was established with the applied field dependence of the blocking temperatures following the de Almeida-Thouless line for the Mn0.6Co0.4Fe2O4 NPs. The shifted hysteresis loops with exchange bias field of 60 Oe and high-field irreversibility up to 60 kOe in FC M- H curve at 10 K show that spin-glass-like surface spins surrounds around ordered core material of the Mn0.6Co0.4Fe2O4 NPs. FMR measurement show that all the TREG-coated Mn x Co1- x Fe2O4 nanoparticles absorb microwave in broad field range of about ten thousands Oe. The spectra for all the samples have broad linewidth because of angular distributions of easy axis and internal fields of nanoparticles.

  13. Surface spin disorder and spin-glass-like behaviour in manganese-substituted cobalt ferrite nanoparticles

    Energy Technology Data Exchange (ETDEWEB)

    Topkaya, R., E-mail: rtopkaya@gyte.edu.tr [Gebze Institute of Technology, Department of Physics (Turkey); Akman, Oe. [Sakarya University, Department of Physics (Turkey); Kazan, S.; Aktas, B. [Gebze Institute of Technology, Department of Physics (Turkey); Durmus, Z.; Baykal, A. [Fatih University, Department of Chemistry (Turkey)

    2012-10-15

    Manganese-substituted cobalt ferrite nanoparticles coated with triethylene glycol (TREG) have been prepared by the glycothermal reaction. The effect of Mn substitution and coating on temperature-dependent magnetic properties of the TREG-coated Mn{sub x}Co{sub 1-x}Fe{sub 2}O{sub 4} nanoparticles (0.0 {<=} x {<=} 0.8) with size of {approx}5-7 nm has been investigated in the temperature range of 10-300 K in a magnetic field up to 9 T. After the irreversible processes of the magnetic hysteresis curves were completed, the high-field regions of these curves were fitted by using a 'law of approach to saturation' to extract the magnetic properties, such as the effective anisotropy constant (K{sub eff}) and the anisotropy field (H{sub A}) etc. High coercive field of 12.6 kOe is observed in pure cobalt ferrite coated with TREG at 10 K. The low temperature unsaturated magnetization behaviour indicates the core-shell structure of the Mn{sub x}Co{sub 1-x}Fe{sub 2}O{sub 4} NPs. Zero-field-cooled (ZFC) and field-cooled (FC) measurements revealed superparamagnetic phase of TREG-coated Mn{sub x}Co{sub 1-x}Fe{sub 2}O{sub 4} nanoparticles at room temperature. The blocking and irreversibility temperatures obtained from ZFC-FC curves decrease at highest Mn concentration (x = 0.8). The existence of spin-glass-like surface layer with freezing temperature of 215 K was established with the applied field dependence of the blocking temperatures following the de Almeida-Thouless line for the Mn{sub 0.6}Co{sub 0.4}Fe{sub 2}O{sub 4} NPs. The shifted hysteresis loops with exchange bias field of 60 Oe and high-field irreversibility up to 60 kOe in FC M-H curve at 10 K show that spin-glass-like surface spins surrounds around ordered core material of the Mn{sub 0.6}Co{sub 0.4}Fe{sub 2}O{sub 4} NPs. FMR measurement show that all the TREG-coated Mn{sub x}Co{sub 1-x}Fe{sub 2}O{sub 4} nanoparticles absorb microwave in broad field range of about ten thousands Oe. The spectra for all the

  14. Single excitation transfer in the quantum regime. A spin-based solid-state approach

    Energy Technology Data Exchange (ETDEWEB)

    Zollitsch, Christoph Wilhelm

    2016-12-02

    Realisation of strong coupling between a superconducting microwave resonator and an ensemble of phosphorus donor spins, contained in an isotopically purified silicon host crystal. Investigation of the dynamical properties of the coupled system at mK temperatures and ultra-low microwave powers. The relaxation and coherence times of the coupled system were extracted by pulsed microwave spectroscopy, with the result that the hybrid system's coherence time is enhanced compared to the uncoupled spin system.

  15. Manipulating charge transfer excited state relaxation and spin crossover in iron coordination complexes with ligand substitution

    DEFF Research Database (Denmark)

    Zhang, Wenkai; Kjær, Kasper Skov; Alonso-Mori, Roberto

    2017-01-01

    ) Kβ hard X-ray fluorescence spectroscopy with femtosecond time-resolved UV-visible absorption spectroscopy to characterize the electronic excited state dynamics initiated by MLCT excitation of [Fe(CN)4(bpy)]2-. The two experimental techniques are highly complementary; the time-resolved UV...

  16. Fast Pulse Measurements and Temperature Variation of Enhanced Magnetic Damping of Spin-Transfer Excitation

    Science.gov (United States)

    Ryan, E. M.; Garcia, A. G. F.; Braganca, P. M.; Fuchs, G. D.; Emley, N. C.; Read, J. C.; Tan, E.; Ralph, D. C.; Buhrman, R. A.; Katine, J. A.

    2007-03-01

    Recently, light terbium (Tb) doping in thin films of permalloy (Py) has been shown to increase the damping parameter α by several orders of magnitude [1]. To directly study the effect of increased α on spin-transfer systems, we have fabricated 0.004 um^2 Py/Cu/Py nanopillar spin valves with 0 and 2% Tb in the free layer, and measured critical currents across a range of temperatures from 4.2 K to 295 K. We find that the critical currents for reversibly switching the free layer, generally expected to be proportional to α, are several times larger on average in the 2% Tb samples than in pure Py samples, and increase linearly with decreasing temperature. We will also discuss FMR data, and data for switching with fast pulses from 1 to 100 nsec at both 150 K and room temperature, along with matching simulations that allows us to extract α and other spin-torque parameters [2]. These results suggest one approach for controllably reducing the negative impact of spin-torque effects on nanoscale spin valve and read head sensors, and achieving a deeper understanding of these spin-torque devices. [1] W. Bailey, P. Kabos, F. Mancoff, and S. E. Russek, IEEE Trans. Magn. 37, 1749 (2001). [2] P. M. Braganca, et al. Appl. Phys. Lett. 87, 112507 (2005).

  17. Surface induces different crystal structures in a room temperature switchable spin crossover compound.

    Science.gov (United States)

    Gentili, Denis; Liscio, Fabiola; Demitri, Nicola; Schäfer, Bernhard; Borgatti, Francesco; Torelli, Piero; Gobaut, Benoit; Panaccione, Giancarlo; Rossi, Giorgio; Degli Esposti, Alessandra; Gazzano, Massimo; Milita, Silvia; Bergenti, Ilaria; Ruani, Giampiero; Šalitroš, Ivan; Ruben, Mario; Cavallini, Massimiliano

    2016-01-01

    We investigated the influence of surfaces in the formation of different crystal structures of a spin crossover compound, namely [Fe(L)2] (LH: (2-(pyrazol-1-yl)-6-(1H-tetrazol-5-yl)pyridine), which is a neutral compound thermally switchable around room temperature. We observed that the surface induces the formation of two different crystal structures, which exhibit opposite spin transitions, i.e. on heating them up to the transition temperature, one polymorph switches from high spin to low spin and the second polymorph switches irreversibly from low spin to high spin. We attributed this inversion to the presence of water molecules H-bonded to the complex tetrazolyl moieties in the crystals. Thin deposits were investigated by means of polarized optical microscopy, atomic force microscopy, X-ray diffraction, X-ray absorption spectroscopy and micro Raman spectroscopy; moreover the analysis of the Raman spectra and the interpretation of spin inversion were supported by DFT calculations.

  18. Observation of Hot Electrons in Surface-Wave Plasmas Excited by Surface Plasmon Polaritons

    Institute of Scientific and Technical Information of China (English)

    HU Ye-Lin; CHEN Zhao-Quan; LIU Ming-Hai; HONG Ling-Li; LI Ping; ZHENG Xiao-Liang; XIA Guang-Qing; HU Xi-Wei

    2011-01-01

    The electron energy distribution functions (EEDFs) are studied in the planar-type surface-wave plasma (SWP)caused by resonant excitation of surface plasmon polaritons (SPPs) using a single cylindrical probe.Sustained plasma characteristics can be considered as a bi-Maxwellian EEDF,which correspond to a superposition of the bulk low-temperature electron and the high-energy electron beam-like part.The beam component energy is pronounced at about 10eV but the bulk part is lower than 3.5eV.The hot electrons included in the proposed plasmas play a significant role in plasma heating and further affect the discharge chemistry.During the past several years,in the fabrication ofamorphous or crystalline silicon films,diamond film synthesis and carbon nanotube growth,the large-area overdense plasma source has been useful.In electronic device fabrication techniques such as etching,ashing or plasma chemical vapor deposition,overdense electrons and radicals are required,especially hot electrons.Among the various plasma devices,the planar-type surface-wave plasma (SWP) source is an advanced plasma source,which is a type of promising plasma source satisfying the above rigorous requirements for large-area plasma processing.%The electron energy distribution functions (EEDFs) are studied in the planar-type surface-wave plasma (SWP) caused by resonant excitation of surface plasmon polaritons (SPPs) using a single cylindrical probe. Sustained plasma characteristics can be considered as a bi-Maxwellian EEDF, which correspond to a superposition of the bulk low-temperature electron and the high-energy electron beam-like part. The beam component energy is pronounced at about 10 eV but the bulk part is lower than 3.5 eV. The hot electrons included in the proposed plasmas play a significant role in plasma heating and further affect the discharge chemistry.

  19. Operator analysis of effective spin-flavor interactions for L=1 excited baryons

    CERN Document Server

    Willemyns, Cintia

    2015-01-01

    We match the non-relativistic quark model, with both flavor dependent and flavor independent effective quark-quark interactions, to the spin-flavor operator basis of the 1/Nc expansion for the L=1 non-strange baryons. We obtain analytic expressions for the coefficients of the 1/Nc operators in terms of radial integrals that depend on the shape and relative strength of the spin-spin, spin-orbit and tensor interactions of the model, which are left unspecified. We obtain several new, parameter-free relations between the seven masses and the two mixing angles that can discriminate between different spin-flavor structures of the effective quark-quark interaction. We discuss in detail how a general parametrization of the mass matrix depends on the mixing angles and is constrained by the assumptions on the effective quark-quark interaction. We find that, within the present experimental uncertainties, consistency with the best values of the mixing angles as determined by a recent global fit to masses and decays does ...

  20. Excitations

    Energy Technology Data Exchange (ETDEWEB)

    Dorner, B. [Institut Max von Laue - Paul Langevin (ILL), 38 - Grenoble (France)

    1996-12-31

    A short introduction to instrumental resolution is followed by a discussion of visibilities of phonon modes due to their eigenvectors. High precision phonon dispersion curves in GaAs are presented together with `ab initio` calculations. Al{sub 2}O{sub 3} is taken as an example of selected visibility due to group theory. By careful determination of phonon intensities eigenvectors can be determined, such as in Silicon and Diamond. The investigation of magnon modes is shown for the garnet Fe{sub 2}Ca{sub 3}(GeO{sub 4}){sub 3}, where also a quantum gap due to zero point spin fluctuations was observed. The study of the splitting of excitons in CsFeCl{sub 3} in an applied magnetic field demonstrates the possibilities of neutron polarisation analysis, which made it possible to observe a mode crossing. An outlook to inelastic X-ray scattering with very high energy resolution of synchrotron radiation is given with the examples of phonons in Beryllium and in water. (author) 19 figs., 36 refs.

  1. Reduced Heat Flux Through Preferential Surface Reactions Leading to Vibrationally and Electronically Excited Product States

    Science.gov (United States)

    2016-03-04

    AFRL-AFOSR-VA-TR-2016-0124 Reduced Heat Flux Through Preferential Surface Reactions Leading to Vibrationally and Electronically Excited Product...Reactions Leading to Vibrationally and Electronically Excited Product States 5a. CONTRACT NUMBER FA9550-12-1-0486 5b. GRANT NUMBER 5c. PROGRAM... Leading to Vibrationally and Electronically Excited Product States FINAL TECHNICAL REPORT: Grant #FA9550-12-1-0486 2013 Basic Research Initiative (BRI

  2. Experimental observation and computational study of the spin-gap excitation in Ba3BiRu2O9

    Science.gov (United States)

    Ling, C. D.; Huang, Z.; Kennedy, B. J.; Rols, S.; Johnson, M. R.; Zbiri, M.; Kimber, S. A. J.; Hudspeth, J.; Adroja, D. T.; Rule, K. C.; Avdeev, M.; Blanchard, P. E. R.

    2016-11-01

    Ba3BiRu2O9 is a 6H-type perovskite compound containing face-sharing octahedral M2O9 (M =Ir , Ru) dimers, which are magnetically frustrated at low temperatures. On cooling through T*=176 K, it undergoes a pronounced magnetostructural transition, which is not accompanied by any change in space group symmetry, long-range magnetic ordering, or charge ordering. Here, we report the first direct evidence from inelastic neutron scattering that this transition is due to an opening of a gap in the excitation spectra of dimers of low-spin Ru4 + (S =1 ) ions. X-ray absorption spectroscopy reveals a change in Ru-Ru orbital overlap at T*, linking the emergence of this spin-gap excitation to the magnetostructural transition. Ab initio calculations point to a geometrically frustrated magnetic ground state due to antiferromagnetic interdimer exchange on a triangular Ru2O9 dimer lattice. X-ray total-scattering data rule out long-range magnetic ordering at low temperatures, consistent with this geometrically frustrated model.

  3. Long-range quantum Ising spin glasses at t=0: gapless collective excitations and universality.

    Science.gov (United States)

    Andreanov, A; Müller, M

    2012-10-26

    We solve the Sherrington-Kirkpatrick model in a transverse field Γ deep in its quantum glass phase at zero temperature. We show that the glass phase is critical everywhere, exhibiting collective excitations with a gapless Ohmic spectral function. Using an effective potential approach, we interpret the latter as arising from disordered collective excitations behaving like weakly coupled, underdamped oscillators. For a small transverse field Γ, the low-frequency spectrum takes a form independent of the fluctuation strength Γ.

  4. Long-Range Quantum Ising Spin Glasses at T=0: Gapless Collective Excitations and Universality

    Science.gov (United States)

    Andreanov, A.; Müller, M.

    2012-10-01

    We solve the Sherrington-Kirkpatrick model in a transverse field Γ deep in its quantum glass phase at zero temperature. We show that the glass phase is critical everywhere, exhibiting collective excitations with a gapless Ohmic spectral function. Using an effective potential approach, we interpret the latter as arising from disordered collective excitations behaving like weakly coupled, underdamped oscillators. For a small transverse field Γ, the low-frequency spectrum takes a form independent of the fluctuation strength Γ.

  5. The surface magnetization study of Cr2O3 by spin polarized low energy electron microscopy

    Science.gov (United States)

    Cao, Shi; Wu, Ning; Zhang, Xin; N'diaye, Alpha; Chen, Gong; Schmid, Andreas; Echtenkamp, Will; Lauter, Valeria; Binek, Christian; Dowben, Peter

    2014-03-01

    The boundary magnetization at the surface of a Cr2O3 single crystal has been demonstrated by using spin-polarized low-energy electron microscopy (SPLEEM), indicating net surface spin polarization. This work shows that the placement of Cr2O3 single crystal in the single domain state, will result in net Cr2O3 spin polarization at the boundary, even in the presence of a gold overlayer. There are indications that the spin-polarized low-energy electron microscopy (SPLEEM) contrast for the two polarizations states is different. In addition, the boundary magnetization protected by the symmetry exists despite of the surface roughness/softness which was studied by the non-spin neutron reflectometry and low energy electron diffraction. Unoccupied surface oxygen sites and chromium sites are possible mechanism contributing to the surface ``softness,'' which will be discussed.

  6. Magnetic excitations in spin-orbital liquid FeSc2S4 in zero and applied magnetic field probed by inelastic neutron scattering

    Science.gov (United States)

    Biffin, Alun; Coldea, Radu; Rüegg, Christian; Zaharko, Oksana; Embs, Jan; Guidi, Tatiana; Tsurkan, Vladimir

    2014-03-01

    In systems where both spin and orbital frustration are present, an intriguing Spin Orbital Liquid (SOL) state is believed to occur where spin and orbital moments remain disordered down to the lowest measurable temperatures. The A-site spinel FeSc2S4 is believed to form such a SOL ground state, with its undistorted cubic structure and diamond lattice of Fe2+ sites providing the ingredients for orbital and spin frustration, respectively. The system displays Curie-Weiss behaviour indicative of strong exchange between S = 2 , L = 2 Fe2+ ions, though it does not order down to the lowest measurable temperatures. Here I will present the results of inelastic, time-of-flight neutron scattering experiments that probe the full bandwidth of the magnetic excitations in a powder sample of FeSc2S4, and provide a consistent model of the observed dynamics in terms of spin-orbital excitations, in both zero-field and in-field measurements. I will discuss in particular how the application of a magnetic field elucidates the spin and orbital nature of these excitations, as the system shows behaviour drastically contrary to its spin-only analogue. We acknowledge support from EPSRC (UK).

  7. Local excitation of surface plasmon polaritons by second-harmonic generation in crystalline organic nanofibers

    DEFF Research Database (Denmark)

    Skovsen, Esben; Søndergaard, Thomas; Fiutowski, Jacek

    2012-01-01

    Coherent local excitation of surface plasmon polaritons (SPPs) by second-harmonic generation (SHG) in aligned crystalline organic functionalized para-phenylene nanofibers deposited on a thin silver film is demonstrated. The excited SPPs are characterized using angle-resolved leakage radiation...

  8. Spin-Free CC2 Implementation of Induced Transitions between Singlet Ground and Triplet Excited States.

    Science.gov (United States)

    Helmich-Paris, Benjamin; Hättig, Christof; van Wüllen, Christoph

    2016-04-12

    In most organic molecules, phosphorescence has its origin in transitions from triplet exited states to the singlet ground state, which are spin-forbidden in nonrelativistic quantum mechanics. A sufficiently accurate description of phosphorescence lifetimes for molecules that contain only light elements can be achieved by treating the spin-orbit coupling (SOC) with perturbation theory (PT). We present an efficient implementation of this approach for the approximate coupled cluster singles and doubles model CC2 in combination with the resolution-of-the-identity approximation for the electron repulsion integrals. The induced oscillator strengths and phosphorescence lifetimes from SOC-PT are computed within the response theory framework. In contrast to previous work, we employ an explicitly spin-coupled basis for singlet and triplet operators. Thereby, a spin-orbital treatment can be entirely avoided for closed-shell molecules. For compounds containing only light elements, the phosphorescence lifetimes obtained with SOC-PT-CC2 are in good agreement with those of exact two-component (X2C) CC2, whereas the calculations are roughly 12 times faster than with X2C. Phosphorescence lifetimes computed for two thioketones with the SOC-PT-CC2 approach agree very well with reference results from experiment and are similar to those obtained with multireference spin-orbit configuration interaction and with X2C-CC2. An application to phosphorescent emitters for metal-free organic light-emitting diodes (OLEDs) with almost 60 atoms and more than 1800 basis functions demonstrates how the approach extends the applicability of coupled cluster methods for studying phosphorescence. The results indicate that other decay channels like vibrational relaxation may become important in such systems if lifetimes are large.

  9. Relative acceleration approach for conduction failure of cardiac excitation propagation on anisotropic curved surfaces

    CERN Document Server

    Chun, Sehun

    2012-01-01

    In cardiac electrophysiology, it is important to predict the necessary conditions for conduction failure, the failure of the cardiac excitation propagation even in the presence of normal excitable tissue, in high-dimensional anisotropic space because these conditions may provide feasible mechanisms for abnormal excitation propagations such as atrial re-entry and, subsequently, atrial fibrillation even without taking into account the time-dependent refractory region. Some conditions of conduction failure have been studied for anisotropy or simple curved surfaces, but the general conditions on anisotropic curved surfaces (anisotropic and curved surface) remain unknown. To predict and analyze conduction failure on anisotropic curved surfaces, a new analytic approach is proposed, called the relative acceleration approach borrowed from spacetime physics. Motivated by a discrete model of cardiac excitation propagation, this approach is based on the hypothesis that a large relative acceleration can translate to a dr...

  10. Enhancement of Smith-Purcell radiation with surface-plasmon excitation

    Institute of Scientific and Technical Information of China (English)

    Zhang Ping; Zhang Ya-Xin; Zhou Jun; Liu Wei-Hao; Zhong Ren-Bin; Liu Sheng-Gang

    2012-01-01

    With the aid of a three-dimensional particle-in-cell code simulation,the enhancement of Smith-Purcell radiation with a surface-plasmon mode excited by a single electron bunch and by a premodulated electron beam is considered in the paper.In the simulation,the model is a grating covered by Ag film.The results demonstrate that when the surface-plasmon mode is excited by a single electron bunch,the maximum radiation occurs at an observation angle depending on the surface-plasmon frequency,and the radiation power can be enhanced more than ten times.And for pre-bunched electron beam excitation,when one of the harmonics of the bunching frequency is resonant with that of the surface-plasmon mode,the radiation power is twenty times more than that from a perfectly conducting grating excited by the same premodulated electron beam.

  11. Excited state surfaces in density functional theory: a new twist on an old problem.

    Science.gov (United States)

    Wiggins, Paul; Williams, J A Gareth; Tozer, David J

    2009-09-07

    Excited state surfaces in density functional theory and the problem of charge transfer are considered from an orbital overlap perspective. For common density functional approximations, the accuracy of the surface will not be uniform if the spatial overlap between the occupied and virtual orbitals involved in the excitation has a strong conformational dependence; the excited state surface will collapse toward the ground state in regions where the overlap is very low. This characteristic is used to predict and to provide insight into the breakdown of excited state surfaces in the classic push-pull 4-(dimethylamino)benzonitrile molecule, as a function of twist angle. The breakdown is eliminated using a Coulomb-attenuated functional. Analogous situations will arise in many molecules.

  12. Low energy nuclear spin excitations in Ho metal investigated by high resolution neutron spectroscopy.

    Science.gov (United States)

    Chatterji, Tapan; Jalarvo, Niina

    2013-04-17

    We have investigated the low energy excitations in metallic Ho by high resolution neutron spectroscopy. We found at T = 3 K clear inelastic peaks in the energy loss and energy gain sides, along with the central elastic peak. The energy of this low energy excitation, which is 26.59 ± 0.02 μeV at T = 3 K, decreased continuously and became zero at TN ≈ 130 K. By fitting the data in the temperature range 100-127.5 K with a power law we obtained the power-law exponent β = 0.37 ± 0.02, which agrees with the expected value β = 0.367 for a three-dimensional Heisenberg model. Thus the energy of the low energy excitations can be associated with the order parameter.

  13. Direct observation of localized dipolar excitations on rough nanostructured surfaces

    DEFF Research Database (Denmark)

    Bozhevolnyi, Sergey I.; Markel, V.A.; Coello, V.;

    1998-01-01

    spatially localized (within 150-250 nm) intensity enhancement by one to two orders of magnitude. These bright light spots are found to be sensitive to the light wavelength, polarization, and angle of incidence. We relate the observed phenomenon to the localization of resonant dipolar excitations in random......Using a photon scanning tunneling microscope (operating alternatively at the wavelengths of 594 and 633 nm) with shear-force feedback we image the topography of silver colloid fractals simultaneously with a near-field intensity distribution. We observe that near-field optical images exhibit...

  14. Investigation of Surface Magnetic Noise by Shallow Spins in Diamond

    NARCIS (Netherlands)

    Rosskopf, T; Dussaux, A; Ohashi, K; Loretz, M; Schirhagl, R; Watanabe, H; Shikata, S; Itoh, KM; Degen, CL

    2014-01-01

    We present measurements of spin relaxation times (T1, T1ρ, T2) on very shallow (≲5  nm) nitrogen-vacancy centers in high-purity diamond single crystals. We find a reduction of spin relaxation times up to 30 times compared to bulk values, indicating the presence of ubiquitous magnetic impurities asso

  15. Fermi surfaces, spin-mixing parameter, and colossal anisotropy of spin relaxation in transition metals from ab initio theory

    Science.gov (United States)

    Zimmermann, Bernd; Mavropoulos, Phivos; Long, Nguyen H.; Gerhorst, Christian-Roman; Blügel, Stefan; Mokrousov, Yuriy

    2016-04-01

    The Fermi surfaces and Elliott-Yafet spin-mixing parameter (EYP) of several elemental metals are studied by ab initio calculations. We focus first on the anisotropy of the EYP as a function of the direction of the spin-quantization axis [B. Zimmermann et al., Phys. Rev. Lett. 109, 236603 (2012), 10.1103/PhysRevLett.109.236603]. We analyze in detail the origin of the gigantic anisotropy in 5 d hcp metals as compared to 5 d cubic metals by band structure calculations and discuss the stability of our results against an applied magnetic field. We further present calculations of light (4 d and 3 d ) hcp crystals, where we find a huge increase of the EYP anisotropy, reaching colossal values as large as 6000 % in hcp Ti. We attribute these findings to the reduced strength of spin-orbit coupling, which promotes the anisotropic spin-flip hot loops at the Fermi surface. In order to conduct these investigations, we developed an adapted tetrahedron-based method for the precise calculation of Fermi surfaces of complicated shape and accurate Fermi-surface integrals within the full-potential relativistic Korringa-Kohn-Rostoker Green function method.

  16. High-field magnetic phase transitions and spin excitations in magnetoelectric LiNiPO4

    DEFF Research Database (Denmark)

    Toft-Petersen, Rasmus; Jensen, Jens; Jensen, Thomas Bagger Stibius;

    2011-01-01

    The magnetically ordered phases and spin dynamics of magnetoelectric LiNiPO4 have been studied in fields up to 17.3 T along the c axis. Using neutron diffraction, we show that a previously proposed linearly polarized incommensurate (IC) structure exists only for temperatures just below the Neel......, the spiral structure is found to lock in to a period of five crystallographic unit cells along the b axis. Based on the neutron-diffraction data, combined with detailed magnetization measurements along all three crystallographic axes, we establish the magnetic phase diagrams for fields up to 17.3 T along c...... the linear and elliptical polarization of the IC structure, and that a generalization of the spin-wave theory, assuming the random-phase approximation, accounts for the inelastic scattering data obtained in the commensurable uniform phase at fields below 12 T as well as those obtained in the high-field IC...

  17. Surface plasmon polariton excitation by second harmonic generation in single organic nanofibers.

    Science.gov (United States)

    Simesen, Paw; Søndergaard, Thomas; Skovsen, Esben; Fiutowski, Jacek; Rubahn, Horst-Günter; Bozhevolnyi, Sergey I; Pedersen, Kjeld

    2015-06-15

    Coherent local excitation of surface plasmon polaritons (SPPs) by second-harmonic generation (SHG) in individual aligned crystalline organic functionalized para-phenylene nanofibers deposited on a thin silver film is demonstrated. The SH-SPP generation is considered theoretically and investigated experimentally with angular-resolved leakage radiation spectroscopy for normal incidence of the excitation beam. Both measurements and simulations show asymmetric excitation of left- and right-propagating SH-SPPs, which is explained as an effect of fiber molecules being oriented at an angle relative to the silver film surface.

  18. Polarization dependence of the spin-density-wave excitations in single-domain chromium

    Energy Technology Data Exchange (ETDEWEB)

    Boeni, P. [Paul Scherrer Inst. (PSI), Villigen (Switzerland); Roessli, B. [Institut Max von Laue - Paul Langevin, 75 - Paris (France); Sternlieb, B.J. [Brookhaven (United States); Lorenzo, E. [Centre National de la Recherche Scientifique (CNRS), 38 - Grenoble (France); Werner, S.A. [Missouri (United States)

    1997-09-01

    A polarized neutron scattering experiment has been performed with a single-Q, single domain sample of chromium in a magnetic field of 4 T. It is confirmed that the longitudinal fluctuations are enhanced for small energy transfers and that the spin wave modes with {delta}S parallel to Q and {delta}S perpendicular to Q are similar. (author) 2 figs., 1 tab., 2 refs.

  19. Triggering of spin-flipping-modulated exchange bias in FeCo nanoparticles by electronic excitation

    Science.gov (United States)

    Sarker, Debalaya; Bhattacharya, Saswata; Srivastava, Pankaj; Ghosh, Santanu

    2016-12-01

    The exchange coupling between ferromagnetic (FM)-antiferromagnetic (AF) interfaces is a key element of modern spintronic devices. We here introduce a new way of triggering exchange bias (EB) in swift heavy ion (SHI) irradiated FeCo-SiO2 films, which is a manifestation of spin-flipping at high irradiation fluence. The elongation of FeCo nanoparticles (NPs) in SiO2 matrix gives rise to perpendicular magnetic anisotropy at intermediate fluence. However, a clear shift in hysteresis loop is evident at the highest fluence. This reveals the existence of an AF exchange pinning domain in the NPs, which is identified not to be oxide shell from XANES analysis. Thermal spike calculations along with first-principles based simulations under the framework of density functional theory (DFT) demonstrate that spin flipping of 3d valence electrons is responsible for formation of these AF domains inside the FM NPs. EXAFS experiments at Fe and Co K-edges further unravel that spin-flipping in highest fluence irradiated film results in reduced bond lengths. The results highlight the possibility of miniaturization of magnetic storage devices by using irradiated NPs instead of conventionally used FM-AF multilayers.

  20. De-excitation of high spin isomers in the sup 1 sup 9 sup 1 Pb isotope

    CERN Document Server

    Lagrange, J M; Dionisio, J S; Vieu, C; Vanhorenbeeck, J

    1999-01-01

    The sup 1 sup 9 sup 1 Pb isotope, produced through different A (b,xn) sup 1 sup 9 sup 1 Pb reactions, where b stands for nuclei such as sup 1 sup 6 O, sup 2 sup 0 Ne, and sup 3 sup 1 P, is studied. The half-life of some excited levels being greater than 10 ns, the recoil catcher method is suitable to look into the de-excitation gamma ray and conversion electron spectra of these states. The conversion coefficients are deduced and e sup - -gamma and gamma-gamma coincidence measurements lead to the part of the level scheme de-exciting these isomers. This level scheme is compared to theoretical predictions obtained through a microscopic calculation in a three quasi-particle approximation, using a surface delta interaction with a reduced pairing component. The conclusions are very similar to those previously obtained for sup 1 sup 9 sup 3 Pb.

  1. Electromagnetic excitation of phonons at C(001) surfaces

    Energy Technology Data Exchange (ETDEWEB)

    Perez-Sanchez, F L [Escuela de Ciencias, Universidad Autonoma ' Benito Juarez' de Oaxaca, Avenida Universidad S/N, Ex-Hacienda de Cinco Senores, Ciudad Universitaria, Oaxaca de Juarez, Oaxaca, 68120 (Mexico); Perez-Rodriguez, F, E-mail: fperez@sirio.ifuap.buap.m [Instituto de Fisica, Benemerita Universidad Autonoma de Puebla, Apartado Post. J-48, Puebla 72570 (Mexico)

    2009-09-02

    The photon-phonon coupling at C(001)-(2 x 1) surfaces and its manifestation in far-infrared reflectance anisotropy spectra (FIR-RAS) are theoretically investigated. We solve the coupled system of equations for the electromagnetic field and lattice vibrations, described within the adiabatic bond charge model (ABCM), with the method of expansion into bulk phonon and photon modes. The calculated FIR-RAS exhibit resonances associated with zone-center surface phonons in good agreement with available HREELS experiments and predictions of vibrational modes for diamond (001)-(2 x 1) surfaces from ABCM and ab initio calculations. Interestingly, the reflectance anisotropy spectra for a C(001)-(2 x 1) surface turn out to be qualitatively different from the spectra for a Si(001)-(2 x 1) surface, reported previously.

  2. Surface waves in a vertically excited circular cylindrical container

    Institute of Scientific and Technical Information of China (English)

    Jian Yong-Jun; E Xue-Quan; Zhang Jie; Meng Jun-Min

    2004-01-01

    The nonlinear free surface amplitude equation, which has been derived from the inviscid fluid by solving the potential equation of water waves with a singular perturbation theory in a vertically oscillating rigid circular cylinder,is investigated successively in the fourth-order Runge-Kutta approach with an equivalent time-step. Computational results include the evolution of the amplitude with time, the characteristics of phase plane determined by the real and imaginary parts of the amplitude, the single-mode selection rules of the surface waves in different forced frequencies,contours of free surface displacement and corresponding three-dimensional evolution of surface waves, etc. In addition,the comparison of the surface wave modes is made between theoretical calculations and experimental measurements,and the results are reasonable although there are some differences in the forced frequency.

  3. Spin excitations in stripe-ordered La{sub 2-x}Sr{sub x}NiO{sub 4} (x=0.275 and ((1)/(3)))

    Energy Technology Data Exchange (ETDEWEB)

    Boothroyd, A.T. E-mail: a.boothroyd1@physics.ox.ac.uk; Freeman, P.G.; Prabhakaran, D.; Woo, H.; Nakajima, K.; Tranquada, J.M.; Yamada, K.; Frost, C.D

    2004-05-01

    We report neutron scattering measurements of the spectrum of magnetic excitations in the stripe-ordered phase of La{sub 2-x}Sr{sub x}NiO{sub 4} (x=0.275 and ((1)/(3))). The propagating spin excitations follow a similar dispersion relation for the two compositions, but the line widths are broader for x=0.275 than for ((1)/(3))

  4. Spin excitations in stripe-ordered La 2- xSr xNiO 4 ( x=0.275 and {1}/{3})

    Science.gov (United States)

    Boothroyd, A. T.; Freeman, P. G.; Prabhakaran, D.; Woo, H.; Nakajima, K.; Tranquada, J. M.; Yamada, K.; Frost, C. D.

    2004-05-01

    We report neutron scattering measurements of the spectrum of magnetic excitations in the stripe-ordered phase of La 2- xSr xNiO 4 ( x=0.275 and {1}/{3}). The propagating spin excitations follow a similar dispersion relation for the two compositions, but the line widths are broader for x=0.275 than for {1}/{3}.

  5. Self-limiting excitation of MEMS devices with surface electrodes

    CERN Document Server

    Kornilovitch, Pavel

    2013-01-01

    An excitation method for MEMS devices with planar electrodes is described. The stationary part of the device (the stator) consists of three electrode arrays arranged in the 'ABCABC' order. 'A', 'B', and 'C' carry time-independent potentials and together form a spatially-periodic electrostatic profile. The moving part of the device (the translator) has two electrode arrays 'ababab', with 'a' and 'b' carrying time-dependent out-of-phase voltages. When the frequency of the time-dependent voltage is close to the natural frequency of the spring-mass system, the translator is driven into resonance. By adjusting the spatial phase of the stationary profile, the driving force on the translator can be maximized for any equilibrium position. Physical misalignment between the stator and translator resulting from imperfect fabrication can be corrected electrically. A dynamical equation describing translator motion is derived and analyzed for resonant and parametric driving. In both cases, the driving force depends on the ...

  6. Quantum dispersion relations for excitations of long folded spinning superstring in AdS_5 x S^5

    CERN Document Server

    Giombi, S; Roiban, R; Tseytlin, A A

    2010-01-01

    We use AdS_5 x S^5 superstring sigma model perturbation theory to compute the leading one-loop corrections to the dispersion relations of the excitations near a long spinning string in AdS. This investigation is partially motivated by the OPE-based approach to the computation of the expectation value of null polygonal Wilson loops suggested in arXiv:1006.2788. Our results are in partial agreement with the recent asymptotic Bethe ansatz computation in arXiv:1010.5237. In particular, we find that the heaviest AdS mode (absent in the ABA approach) is stable and has a corrected one-loop dispersion relation similar to the other massive modes. Its stability might hold also at the next-to-leading order as we suggest using a unitarity-based argument.

  7. Extensive spin-orbit multi-reference computations on the excited states of the phosphorus monochloride molecule

    Science.gov (United States)

    Zhang, Xiaomei; Yan, Peiyuan; Li, Rui; Gai, Zhiqiang; Liang, Guiying; Xu, Haifeng; Yan, Bing

    2016-09-01

    Total 34 Λ-S states of the PCl molecule have been studied by using the multi-reference configuration interaction plus the Davidson correction (MRCI+Q) method with the correlation consistent quadruple-zeta quality basis set. These states are correlated to three dissociation limits P(4Su)+Cl(2Pu), P(2Du)+Cl(2Pu), and P(2Pu)+Cl(2Pu), respectively. The potential energy curves (PECs) of the Λ-S states have been calculated, from which the spectroscopic constants of the bound states are determined. The calculated spectroscopic results well reproduce the available measurements. The spin-orbit matrix elements between the Λ-S states have been calculated, which indicate that the perturbations exist in the interacting system 11Π-23Π and 11Π-23Σ-. And the excited a1Δ, b1Σ+, 21Σ+ states could be predissociated induced by the spin-orbit coupling (SOC) effect. The SOC calculation on the PCl molecule has been performed with the state interaction method. This is the first time that the SOC effect of the PCl has been studied theoretically. The SOC effect leads to the 34 Λ-S states split into the 74 Ω states. The ground state X3Σ- splits into the X3 Σ0-+ (X10+) and X3Σ1- (X21) states. For the zero-field splitting of the X3Σ- state, the spin-orbit contribution of 6 cm-1 is much larger than spin-spin contribution of 0.32 cm-1. Under the influence of the SOC effect, the spectroscopic results of the a1Δ and b1Σ+ states have very small changes, but the dissociation energies strongly decrease. The transition properties of PCl are also predicted, including the E1, M1, and E2 transition moments, the Franck-Condon factors, the transition probabilities, and the radiative lifetimes. For the transitions from a1Δ-X3Σ- and b1Σ+-X3Σ-, the transition probabilities are in order of AE1 > AM1 ≫ AE2. The lifetimes for the b1Σ+(v'=0) state are 4.87ms (E1) and 4.57 ms (E1+M1), in good agreement with the available experimental result of 4.9±0.8 ms.

  8. High spin spectroscopy near the N=Z line: Channel selection and excitation energy systematics

    Energy Technology Data Exchange (ETDEWEB)

    Svensson, C.E.; Cameron, J.A.; Flibotte, S. [McMaster Univ., Ontario (Canada)] [and others

    1996-12-31

    The total {gamma}-ray and charged-particle energies emitted in fusion-evaporation reactions leading to N=Z compound systems in the A = 50-70 mass region have been measured with the 8{pi} {gamma}-ray spectrometer and the miniball charged-particle detector array. A new method of channel selection has been developed which combines particle identification with these total energy measurements and greatly improves upon the selectivity possible with particle detection alone. In addition, the event by event measurement of total {gamma}-ray energies using the BGO ball of the 8{pi} spectrometer has allowed a determination of excitation energies following particle evaporation for a large number of channels in several different reactions. The new channel selection procedure and excitation energy systematics are illustrated with data from the reaction of {sup 24}Mg on {sup 40}Ca at E{sub lab} = 80MeV.

  9. Hyper Open-Shell States: The Lowest Excited Spin States of O Atom, Fe(2+) Ion, and FeF2.

    Science.gov (United States)

    Varga, Zoltan; Verma, Pragya; Truhlar, Donald G

    2017-09-13

    Excited spin states are important for reactivity, catalysis, and magnetic applications. This work examines the relative energies of the spin states of O atom, Fe(2+) ion, and FeF2 and characterizes their excited spin states. Both single-configuration and multireference methods are used to establish the character of the lowest singlet excited state of all three systems and the lowest triplet excited state of Fe(2+) and FeF2. We find that the conventional representation of the orbital occupancies is incorrect in that the states have more unpaired electrons than the minimum number required by their total electron spin quantum number. In particular, we find that, for a given spin state, an electronic configuration with more than 2S unpaired electrons is more stable than the configuration with 2S unpaired electrons (where S is the spin of the system). For instance, triplet FeF2 with four unpaired electrons is lower in energy than triplet FeF2 with two unpaired electrons. Such highly open-shell configurations are labeled as hyper open-shell electronic configurations in this work and are compared to ordinary open-shell or closed-shell electronic configurations. The hyper open-shell states considered in this work are especially interesting because, unlike typical biradicals and polyradicals, the unpaired electrons are all on the same center. This work shows that the conventional perspective on spin-state energetics that usually assumes ordinary open shells for single-centered radicals needs modification to take into account, whenever possible, hyper open-shell configurations as well.

  10. Dynamic Spin Rig Upgraded With a Five- Axis-Controlled Three-Magnetic-Bearing Support System With Forward Excitation

    Science.gov (United States)

    Morrison, Carlos R.; Mehmed, Oral

    2003-01-01

    The NASA Glenn Research Center Dynamic Spin Rig is used for experimental evaluation of vibration analysis methods and dynamic characteristics for rotating systems. Measurements are made while rotors are spun and vibrated in a vacuum chamber. The rig has been upgraded with a new active magnetic bearing rotor support and excitation system. This design is expected to provide operational improvements over the existing rig. The rig will be able to be operated in either the old or new configuration. In the old configuration, two ball bearings support the vertical shaft of the rig, with the test article located between the bearings. Because the bearings operate in a vacuum, lubrication is limited to grease. This limits bearing life and speed. In addition, the old configuration employs two voice-coil electromagnetic shakers to apply oscillatory axial forces or transverse moments to the rotor shaft through a thrust bearing. The excitation amplitudes that can be imparted to the test article with this system are not adequate for components that are highly damped. It is expected that the new design will overcome these limitations.

  11. Direct observation of low energy nuclear spin excitations in HoCrO3 by high resolution neutron spectroscopy.

    Science.gov (United States)

    Chatterji, T; Jalarvo, N; Kumar, C M N; Xiao, Y; Brückel, Th

    2013-07-17

    We have investigated low energy nuclear spin excitations in the strongly correlated electron compound HoCrO3. We observe clear inelastic peaks at E = 22.18 ± 0.04 μeV in both energy loss and gain sides. The energy of the inelastic peaks remains constant in the temperature range 1.5-40 K at which they are observed. The intensity of the inelastic peak increases at first with increasing temperature and then decreases at higher temperatures. The temperature dependence of the energy and intensity of the inelastic peaks is very unusual compared to that observed in other Nd, Co, V and also simple Ho compounds. Huge quasielastic scattering appears at higher temperatures presumably due to the fluctuating electronic moments of the Ho ions that get increasingly disordered at higher temperatures. The strong quasielastic scattering may also originate in the first Ho crystal-field excitations at about 1.5 meV.

  12. Spin to Charge Interconversion Phenomena in the Interface and Surface States

    Science.gov (United States)

    Ando, Yuichiro; Shiraishi, Masashi

    2017-01-01

    In 1985, Johnson and Silsbee realized the creation of a spin current in nonmagnetic metals, which inspired a vast number of studies related to the spin current until now. Creation of the spin current has been realized in metals, semiconductors, and insulators to date and has provided a fruitful research field. Spin-dependent conductance and spin torque paved a new way for spintronic application, and highly efficient interconversion between spin information and an industrially used one, such as charge current, light, magnetic moment and heat current, became a central topic. In the early stage, the main field of such interconversion was bulk materials; the focus then gradually shifted to surface and interface states. The properties of surface and interface states became pronounced in nanoscale spintronics devices, and a variety of functions have been realized at the interface between two materials, enabling limitless possibilities for spin functions. This review provides an overview of the recent progress of the spin-charge interconversion in the surface and interface states. We also introduce several spurious effects that should be paid careful attention for quantitative investigations.

  13. Nearly three orders of magnitude enhancement of Goos-Hanchen shift by exciting Bloch surface wave.

    Science.gov (United States)

    Wan, Yuhang; Zheng, Zheng; Kong, Weijing; Zhao, Xin; Liu, Ya; Bian, Yusheng; Liu, Jiansheng

    2012-04-09

    Goos-Hanchen effect is experimentally studied when the Bloch surface wave is excited in the forbidden band of a one-dimensional photonic band-gap structure. By tuning the refractive index of the cladding covering the truncated photonic crystal structure, either a guided or a surface mode can be excited. In the latter case, strong enhancement of the Goos-Hanchen shift induced by the Bloch-surface-wave results in sub-millimeter shifts of the reflected beam position. Such giant Goos-Hanchen shift, ~750 times of the wavelength, could enable many intriguing applications that had been less than feasible to implement before.

  14. Possible surface plasmon polariton excitation under femtosecond laser irradiation of silicon

    Energy Technology Data Exchange (ETDEWEB)

    Derrien, Thibault J.-Y. [Laboratoire Hubert Curien (LabHC), UMR CNRS 5516 - Université Jean-Monnet. Bâtiment F, 18 rue du Professeur Benoit Lauras, F-42000 Saint-Etienne (France); Laboratoire Lasers, Plasmas et Procédés Photoniques (LP3), UMR CNRS 7341 - Aix-Marseille Université, Parc Technologique et Scientifique de Luminy, Case 917, 163 avenue de Luminy, F-13288 Marseille Cedex 09 (France); Itina, Tatiana E. [Laboratoire Hubert Curien (LabHC), UMR CNRS 5516 - Université Jean-Monnet. Bâtiment F, 18 rue du Professeur Benoit Lauras, F-42000 Saint-Etienne (France); Torres, Rémi; Sarnet, Thierry; Sentis, Marc [Laboratoire Lasers, Plasmas et Procédés Photoniques (LP3), UMR CNRS 7341 - Aix-Marseille Université, Parc Technologique et Scientifique de Luminy, Case 917, 163 avenue de Luminy, F-13288 Marseille Cedex 09 (France)

    2013-08-28

    The mechanisms of ripple formation on silicon surface by femtosecond laser pulses are investigated. We demonstrate the transient evolution of the density of the excited free-carriers. As a result, the experimental conditions required for the excitation of surface plasmon polaritons are revealed. The periods of the resulting structures are then investigated as a function of laser parameters, such as the angle of incidence, laser fluence, and polarization. The obtained dependencies provide a way of better control over the properties of the periodic structures induced by femtosecond laser on the surface of a semiconductor material.

  15. Spin polarized surface resonance bands in single layer Bi on Ge(1 1 1)

    Science.gov (United States)

    Bottegoni, F.; Calloni, A.; Bussetti, G.; Camera, A.; Zucchetti, C.; Finazzi, M.; Duò, L.; Ciccacci, F.

    2016-05-01

    The spin features of surface resonance bands in single layer Bi on Ge(1 1 1) are studied by means of spin- and angle-resolved photoemission spectroscopy and inverse photoemission spectroscopy. We characterize the occupied and empty surface states of Ge(1 1 1) and show that the deposition of one monolayer of Bi on Ge(1 1 1) leads to the appearance of spin-polarized surface resonance bands. In particular, the C 3v symmetry, which Bi adatoms adopt on Ge(1 1 1), allows for the presence of Rashba-like occupied and unoccupied electronic states around the \\overline{\\text{M}} point of the Bi surface Brillouin zone with a giant spin-orbit constant |{α\\text{R}}| =≤ft(1.4+/- 0.1\\right) eV · Å.

  16. Persistent coherence and spin polarization of topological surface states on topological insulators

    Science.gov (United States)

    Pan, Z.-H.; Vescovo, E.; Fedorov, A. V.; Gu, G. D.; Valla, T.

    2013-07-01

    Gapless surface states on topological insulators are protected from elastic scattering on nonmagnetic impurities, which makes them promising candidates for low-power electronic applications. However, for widespread applications, these states should remain coherent and significantly spin polarized at ambient temperatures. Here, we studied the coherence and spin structure of the topological states on the surface of a model topological insulator, Bi2Se3, at elevated temperatures in spin- and angle-resolved photoemission spectroscopy. We found an extremely weak broadening and essentially no decay of spin polarization of the topological surface state up to room temperature. Our results demonstrate that the topological states on surfaces of topological insulators could serve as a basis for room-temperature electronic devices.

  17. Giant enhancement of sum-frequency generation upon excitation of a surface plasmon-polariton

    NARCIS (Netherlands)

    Alieva, E. V.; Petrov, Y. E.; Yakovlev, V. A.; Eliel, E. R.; van der Ham, E. W. M.; Vrehen, Q. H. F.; van der Meer, A. F. G.; Sychugov, V. A.

    1997-01-01

    The generation of the sum frequency of visible (0.5235 mu m) and IP (10 mu m) radiation on smooth and corrugated silver surfaces is investigated. The sum-frequency signal obtained with a visible-range surface plasmon-polariton excited on a corrugated silver-air interface is found to be more than

  18. Surface plasmon polariton excitation by second harmonic generation in single organic nanofibers

    DEFF Research Database (Denmark)

    Simesen, Paw; Søndergaard, Thomas; Skovsen, Esben

    2015-01-01

    Coherent local excitation of surface plasmon polaritons (SPPs) by second-harmonic generation (SHG) in individual aligned crystalline organic functionalized para-phenylene nanofibers deposited on a thin silver film is demonstrated. The SH-SPP generation is considered theoretically and investigated...... to the silver film surface....

  19. SAW devices based on novel surface wave excitations

    Science.gov (United States)

    Therrien, Joel; Dai, Lian

    2015-03-01

    Surface Acoustic Wave (SAW) devices have applications in radio frequency and microwave filtering as well as highly sensitive sensors. Current SAW design employs the use of an array of electrode pairs, referred to as Inter-Digitated Transducers (IDTs) for creating and receiving surface waves on piezoelectric substrates. The pitch of the electrode pairs along with the properties of the substrate determine the operating frequency. The number of electrode pairs determine the bandwidth of the emitted waves. We will present a novel configuration that eliminates the need for the IDTs and replaces with with a single circular electrode located inside a larger ground ring. This configuration induces drumhead modes. We will show that the resonant frequencies follow the zeros of Bessel functions of the first kind. Applications in RF filtering and mass sensing will be presented.

  20. Ligand manipulation of charge transfer excited state relaxation and spin crossover in [Fe(2,2′-bipyridine)2(CN)2

    Science.gov (United States)

    Kjær, Kasper S.; Zhang, Wenkai; Alonso-Mori, Roberto; Bergmann, Uwe; Chollet, Matthieu; Hadt, Ryan G.; Hartsock, Robert W.; Harlang, Tobias; Kroll, Thomas; Kubiček, Katharina; Lemke, Henrik T.; Liang, Huiyang W.; Liu, Yizhu; Nielsen, Martin M.; Robinson, Joseph S.; Solomon, Edward I.; Sokaras, Dimosthenis; van Driel, Tim B.; Weng, Tsu-Chien; Zhu, Diling; Persson, Petter; Wärnmark, Kenneth; Sundström, Villy; Gaffney, Kelly J.

    2017-01-01

    We have used femtosecond resolution UV-visible and Kβ x-ray emission spectroscopy to characterize the electronic excited state dynamics of [Fe(bpy)2(CN)2], where bpy=2,2′-bipyridine, initiated by metal-to-ligand charge transfer (MLCT) excitation. The excited-state absorption in the transient UV-visible spectra, associated with the 2,2′-bipyridine radical anion, provides a robust marker for the MLCT excited state, while the transient Kβ x-ray emission spectra provide a clear measure of intermediate and high spin metal-centered excited states. From these measurements, we conclude that the MLCT state of [Fe(bpy)2(CN)2] undergoes ultrafast spin crossover to a metal-centered quintet excited state through a short lived metal-centered triplet transient species. These measurements of [Fe(bpy)2(CN)2] complement prior measurement performed on [Fe(bpy)3]2+ and [Fe(bpy)(CN)4]2− in dimethylsulfoxide solution and help complete the chemical series [Fe(bpy)N(CN)6–2N]2N-4, where N = 1–3. The measurements confirm that simple ligand modifications can significantly change the relaxation pathways and excited state lifetimes and support the further investigation of light harvesting and photocatalytic applications of 3d transition metal complexes. PMID:28653021

  1. Spinon Fermi surface U (1 ) spin liquid in the spin-orbit-coupled triangular-lattice Mott insulator YbMgGaO4

    Science.gov (United States)

    Li, Yao-Dong; Lu, Yuan-Ming; Chen, Gang

    2017-08-01

    Motivated by the recent progress in the spin-orbit-coupled triangular lattice spin liquid candidate YbMgGaO4, we carry out a systematic projective symmetry group analysis and mean-field study of candidate U (1 ) spin-liquid ground states. Due to the spin-orbital entanglement of the Yb moments, the space-group symmetry operation transforms both the position and the orientation of the local moments, and hence it brings different features for the projective realization of the lattice symmetries from the cases with spin-only moments. Among the eight U (1 ) spin liquids that we find with the fermionic parton construction, only one spin-liquid state, which was proposed and analyzed by Yao Shen et al. [Nature (London) 540, 559 (2016), 10.1038/nature20614] and labeled as U1A00 in the present work, stands out and gives a large spinon Fermi surface and provides a consistent explanation for the spectroscopic results in YbMgGaO4. Further connection of this spinon Fermi surface U (1 ) spin liquid with YbMgGaO4 and the future directions are discussed. Finally, our results may apply to other spin-orbit-coupled triangular lattice spin-liquid candidates, and more broadly, our general approach can be well extended to spin-orbit-coupled spin-liquid candidate materials.

  2. Surface plasmon excitation and manipulation in disordered two-dimmensional nanoparticle arrays

    DEFF Research Database (Denmark)

    Coello, Victor; Cortes, Rodolfo; García Ortíz, César Eduardo

    2013-01-01

    We present experimental and numerical results of simultaneous surface plasmon polariton (SPP) excitation and in-plane manipulation with random arrays of gold nanoparticles. The recorded images were obtained by using leakage radiation microscopy (LRM) for the excitation wavelength of 633 nm...... and for di®erent densities of particles. The numerical model makes use of a composed analytic Green dyadic which takes into account near- and far-¯eld regions, with the latter being approximated by the part describing the scattering via excitation of SPP. The LRM optical images obtained are related...

  3. Perfect optical vortex enhanced surface plasmon excitation for plasmonic structured illumination microscopy imaging

    Science.gov (United States)

    Zhang, Chonglei; Min, Changjun; Du, Luping; Yuan, X.-C.

    2016-05-01

    We propose an all-optical technique for plasmonic structured illumination microscopy (PSIM) with perfect optical vortex (POV). POV can improve the efficiency of the excitation of surface plasma and reduce the background noise of the excited fluorescence. The plasmonic standing wave patterns are excited by POV with fractional topological charges for accurate phase shift of {-2π/3, 0, and 2π/3}. The imaging resolution of less than 200 nm was produced. This PSIM technique is expected to be used as a wide field, super resolution imaging technique in dynamic biological imaging.

  4. Amplitude and phase of surface plasmon polaritons excited at a step edge

    DEFF Research Database (Denmark)

    Klick, Alwin; de la Cruz, Sergio; Lemke, Christoph

    2016-01-01

    A combined experimental and theoretical study on the laser-induced excitation of surface plasmon polaritons (SPP) at well-defined step edges of a gold–vacuum interface is presented. As a relevant parameter determining the coupling efficiency between laser field and SPP, we identify the ratio...... between step height h and excitation wavelength λ. For specific values of h/λ, an almost complete suppression of SPP excitation is observed, which corresponds to a condition of constructive interference between the waves reflected at the top and bottom of the step. Experiment and theory show, furthermore...

  5. A variational surface hopping algorithm for the sub-Ohmic spin-boson model

    CERN Document Server

    Yao, Yao

    2013-01-01

    The Davydov D1 ansatz, which assigns an individual bosonic trajectory to each spin state, is an efficient, yet extremely accurate trial state for time-dependent variation of the the sub-Ohmic spin-boson model [J. Chem. Phys. 138, 084111 (2013)]. A surface hopping algorithm is developed employing the Davydov D1 ansatz to study the spin dynamics with a sub-Ohmic bosonic bath. The algorithm takes into account both coherent and incoherent dynamics of the population evolution in a unified manner, and compared with semiclassical surface hopping algorithms, hopping rates calculated in this work follow more closely the Marcus formula.

  6. Direct observation of spin-resolved full and empty electron states in ferromagnetic surfaces

    Energy Technology Data Exchange (ETDEWEB)

    Berti, G., E-mail: giulia.berti@polimi.it; Calloni, A.; Brambilla, A.; Bussetti, G.; Duò, L.; Ciccacci, F. [Dipartimento di Fisica, Politecnico di Milano, Piazza Leonardo da Vinci 32, I-20133, Milano (Italy)

    2014-07-15

    We present a versatile apparatus for the study of ferromagnetic surfaces, which combines spin-polarized photoemission and inverse photoemission spectroscopies. Samples can be grown by molecular beam epitaxy and analyzed in situ. Spin-resolved photoemission spectroscopy analysis is done with a hemispherical electron analyzer coupled to a 25 kV-Mott detector. Inverse photoemission spectroscopy experiments are performed with GaAs crystals as spin-polarized electron sources and a UV bandpass photon detector. As an example, measurements on the oxygen passivated Fe(100)-p(1×1)O surface are presented.

  7. Excitation of exciton states on a curved surface

    Science.gov (United States)

    Silotia, Poonam; Prasad, Vinod

    2016-05-01

    Excitonic transitions on the surface of a sphere have been studied in he presence of external static electric and laser fields. The spectrum and the various coupling matrix elements, (for n = 1 , 2 , 3), between few states of exciton have been evaluated in the absence and presence of excitonic Coulombic interaction with different values of dielectric constant. Variation of various physical quantities: energy eigenvalues, transition probability, orientational and alignment parameter, has been shown to have strong dependence on the laser field and static electric field.

  8. Spin Coherence at the Nanoscale: Polymer Surfaces and Interfaces

    Energy Technology Data Exchange (ETDEWEB)

    Epstein, Arthur J. [Professor

    2013-09-10

    Breakthrough results were achieved during the reporting period in the areas of organic spintronics. (A) For the first time the giant magnetic resistance (GMR) was observed in spin valve with an organic spacer. Thus we demonstrated the ability of organic semiconductors to transport spin in GMR devices using rubrene as a prototype for organic semiconductors. (B) We discovered the electrical bistability and spin valve effect in a ferromagnet /organic semiconductor/ ferromagnet heterojunction. The mechanism of switching between conducting phases and its potential applications were suggested. (C) The ability of V(TCNE)x to inject spin into organic semiconductors such as rubrene was demonstrated for the first time. The mechanisms of spin injection and transport from and into organic magnets as well through organic semiconductors were elucidated. (D) In collaboration with the group of OSU Prof. Johnston-Halperin we reported the successful extraction of spin polarized current from a thin film of the organic-based room temperature ferrimagnetic semiconductor V[TCNE]x and its subsequent injection into a GaAs/AlGaAs light-emitting diode (LED). Thus all basic steps for fabrication of room temperature, light weight, flexible all organic spintronic devices were successfully performed. (E) A new synthesis/processing route for preparation of V(TCNE)x enabling control of interface and film thicknesses at the nanoscale was developed at OSU. Preliminary results show these films are higher quality and what is extremely important they are substantially more air stable than earlier prepared V(TCNE)x. In sum the breakthrough results we achieved in the past two years form the basis of a promising new technology, Multifunctional Flexible Organic-based Spintronics (MFOBS). MFOBS technology enables us fabrication of full function flexible spintronic devices that operate at room temperature.

  9. Spin- and angle-resolved photoemission spectroscopy study of the Au(1 1 1) Shockley surface state

    Energy Technology Data Exchange (ETDEWEB)

    Muntwiler, Matthias E-mail: m.muntwiler@physik.unizh.ch; Hoesch, Moritz; Petrov, Vladimir N.; Hengsberger, Matthias; Patthey, Luc; Shi Ming; Falub, Mihaela; Greber, Thomas; Osterwalder, Juerg

    2004-07-01

    The spin character of the splitting of the Shockley surface state on Au(111) is directly verified by measurements of the in-plane and out-of-plane spin polarizations in angle-resolved photoemission spectra. The two parabolic sub-bands that are momentum-shifted with respect to each other, reveal a distinct, opposite spin polarization that within the errors lies in the surface plane. The measured in-plane orientation of the spin vectors is consistent with the simple spin structure expected from a nearly-free-electron model, where the polarization axis is tangential to the Fermi surface of the surface state.

  10. A spiral plasmonic lens with directional excitation of surface plasmons.

    Science.gov (United States)

    Guo, Qingrui; Zhang, Chi; Hu, Xinhua

    2016-08-26

    Conventional plasmonic lenses are composed of curved slits carved through metallic films. Here, we propose a new plasmonic lens based on a metallic slit with an auxiliary groove. When the lens is illumined normally, only inward surface plasmon polaritons (SPPs) can be generated and then focused into a hot spot at the center of the lens. The focusing effect is theoretically investigated by varying the groove parameters and incident polarizations. It is found that this phenomenon exists for both the circular and linear polarizations of incidence. Under optimal groove parameters, the intensity of the focal spot in our lens can be 2.5 times of that in one without grooves for both linearly and circularly polarized illuminations.

  11. Surface-Mediated Solidification of a Semiconducting Polymer during Time-Controlled Spin-Coating.

    Science.gov (United States)

    Na, Jin Yeong; Kang, Boseok; Lee, Seung Goo; Cho, Kilwon; Park, Yeong Don

    2016-12-29

    Spin-casting a polymer semiconductor solution over a short period of only a few seconds dramatically improved the molecular ordering and charge transport properties of the resulting semiconductor thin films. In this process, it was quite important to halt spinning before the drying line propagation had begun. Here, we elucidated the effects of the substrate surface characteristics on the drying kinetics during spin-coating, systematically investigated the microstructural evolution during semiconducting polymer solidification, and evaluated the performances of the resulting polymer field-effect transistors. We demonstrated that the spin time required to enhance the molecular ordering and electrical properties of the polythiophene thin films was strongly correlated with the solidification onset time, which was altered by surface treatments introduced onto the substrate surfaces.

  12. Influence of optical coherence on the electron spin in singly charged InP quantum dots excited by resonant laser pulses

    Science.gov (United States)

    Tomimoto, Shinichi; Kawana, Keisuke; Murakami, Akira; Masumoto, Yasuaki

    2012-06-01

    We have experimentally studied the spin dynamics of excitons, electrons, and trions in charge-tunable InP/InGaP quantum dots (QDs) excited by picosecond resonant laser pulses by observing the time-resolved Kerr rotation. In singly charged QDs, inversion of the spin polarization direction of doped electrons is found to be caused simply by variation in the pulse intensity, which is accompanied by an abrupt change of the spin coherence time. This phenomenon is reproduced by density-matrix calculations allowing for the reaction on the QD electron-trion four-level system during its coherent radiation emission. This result means that the optical coherence is another critical factor affecting electron spin coherence.

  13. Effect of surface tension on the mode selection of vertically excited surface waves in a circular cylindrical vessel

    Institute of Scientific and Technical Information of China (English)

    Jian Yong-Jun; E Xue-Quan; Zhang Jie; Meng Jun-Min

    2004-01-01

    Singular perturbation theory of two-time-scale expansions was developed in inviscid fluids to investigate patternforming, structure of the single surface standing wave, and its evolution with time in a circular cylindrical vessel subject to a vertical oscillation. A nonlinear slowly varying complex amplitude equation, which involves a cubic nonlinear term,an external excitation and the influence of surface tension, was derived from the potential flow equation. Surface tension was introduced by the boundary condition of the free surface in an ideal and incompressible fluid. The results show that when forced frequency is low, the effect of surface tension on the mode selection of surface waves is not important.However, when the forced frequency is high, the surface tension cannot be neglected. This manifests that the function of surface tension is to cause the free surface to return to its equilibrium configuration. In addition, the effect of surface tension seems to make the theoretical results much closer to experimental results.

  14. Hosting of surface states in spin-orbit induced projected bulk band gaps of W(1 1 0) and Ir(1 1 1)

    Science.gov (United States)

    Elmers, H. J.; Kutnyakhov, D.; Chernov, S. V.; Medjanik, K.; Fedchenko, O.; Zaporozhchenko-Zymakova, A.; Ellguth, M.; Tusche, C.; Viefhaus, J.; Schönhense, G.

    2017-06-01

    Spin-momentum locking of surface states has attracted great interest in recent years due to envisioned technological applications in the field of spintronics. Normal metal surfaces like W(1 1 0) and Ir(1 1 1) show surface states with energy dispersions and spin-polarization textures, which are reminiscent of topologically non-trivial surface states. In order to understand this phenomenon the connection of bulk and surface states has to be explored. Using time-of-flight momentum microscopy with soft x-ray excitation, we present a comprehensive analysis of the bulk bands of W and Ir. Surface states are determined by the same method with photon excitation in the vacuum ultraviolet region. The superposition of both spectral densities reveals the hosting of surface states within the gap structure of bulk bands projected on the surface Brillouin zone. Quantitative differences in the extension of experimental and theoretical local band gaps indicate an underestimation of electron correlation effects in theory.

  15. An improved model electronic Hamiltonian for potential energy surfaces and spin-orbit couplings of low-lying d-d states of [Fe(bpy)3]2+.

    Science.gov (United States)

    Iuchi, Satoru; Koga, Nobuaki

    2014-01-14

    With the aim of exploring excited state dynamics, a model electronic Hamiltonian for several low-lying d-d states of [Fe(bpy)3](2+) complex [S. Iuchi, J. Chem. Phys. 136, 064519 (2012)] is refined using density-functional theory calculations of singlet, triplet, and quintet states as benchmarks. Spin-orbit coupling elements are also evaluated within the framework of the model Hamiltonian. The accuracy of the developed model Hamiltonian is determined by examining potential energies and spin-orbit couplings at surface crossing regions between different spin states. Insights into the potential energy surfaces around surface crossing regions are also provided through molecular dynamics simulations. The results demonstrate that the constructed model Hamiltonian can be used for studies on the d-d excited state dynamics of [Fe(bpy)3](2+).

  16. Surface-catalyzed recombination into excited electronic, vibrational, rotational, and kinetic energy states: A review

    Science.gov (United States)

    Kofsky, I. L.; Barrett, J. L.

    1985-01-01

    Laboratory experiments in which recombined CO, CO2, D2O, OH, N2, H2, and O2 molecules desorb from surfaces in excited internal and translational states are briefly reviewed. Unequilibrated distributions predominate from the principally catalytic metal substrates so far investigated. Mean kinetic energies have been observed up to approx. 3x, and in some cases less than, wall-thermal; the velocity distributions generally vary with emission angle, with non-Lambertian particle fluxes. The excitation state populations are found to depend on surface impurities, in an as yet unexplained way.

  17. Local excitation of surface plasmon polaritons using nitrogen-vacancy centers

    CERN Document Server

    Garcia-Ortiz, Cesar E; Bozhevolnyi, Sergey I

    2016-01-01

    Surface plasmon polaritons (SPPs) are locally excited at silver surfaces using (~100) nm-sized nanodiamonds (NDs) with multiple nitrogen-vacancy (NV) centers (~400). The fluorescence from an externally illuminated (at 532 nm) ND and from nearby NDs, which are not illuminated but produce out-of-plane scattering of SPPs excited by the illuminated ND, exhibit distinctly different wavelength spectra, showing short-wavelength filtering due to the SPP propagation loss. The results indicate that NDs with multiple NV centers can be used as efficient sub-wavelength SPP sources in planar integrated plasmonics for various applications.

  18. Etats excites en couche interne de haut spin de neon hautement ionise

    Science.gov (United States)

    Lapierre, Alain

    En plus d'être observés lors de plusieurs phénomènes d'interactions multi- électroniques et multi-atomiques, la description des états excités en couche interne est un test sensible à celle de la corrélation électronique. Suivant une spectroscopie faisceau- lame effectuée antérieurement des régions spectrales de l'ultraviolet et du visible (1800-5300 Å) de néon à 10 MeV, des raies spectrales (d'émission) satellites de celles des transitions hydrogéniques (l = n - 1) et l < n - 1, n = 6 - n' = 7, n = 7 - n' = 8 et n = 8 - n' = 9 du néon lithiumoïde (Ne VIII) sont assignées à l'aide de calculs Hartree-Fock, à des transitions de mêmes nombres quantiques principaux entre des états quadruplet dont le cœur est excité en 1s2s 3S. Quelques raies sont assignées à des transitions entre des niveaux n = 3 pour le Ne VI, VII et IX. Par la suite, les transitions quadruplet, quintuplet et sextuplet n = 2 - n' = 3 et n = 2 - n' = 4 du néon lithiumoïde, bérylliumoïde (Ne VII) et boroïde (Ne VI), respectivement, ont été investiguées par spectroscopie faisceau-lame dans la région spectrale des XUV (60-125 Å). Ces investigations sont supportées par des calculs Hartree-Fock et des régressions linéaires sur les séquences isoélectroniques, effectués en parallèle. Des mesures de la durée de vie moyenne de termes n = 3 ont été réalisées et plusieurs raies sont nouvellement identifiées à des transitions de Ne VI à IX.

  19. CAPILLARY EFFECT ON VERTICALLY EXCITED SURFACE WAVE IN CIRCULAR CYLINDRICAL VESSEL

    Institute of Scientific and Technical Information of China (English)

    JIAN Yong-jun; E Xue-quan; ZHANG Jie

    2006-01-01

    In a vertically oscillating circular cylindrical container, singular perturbation theory of two-time scale expansions was developed in inviscid fluids to investigate the motion of single free surface standing wave including the effect of surface tension. A nonlinear slowly varying amplitude equation, which incorporates cubic nonlinear term,external excitation and the influence of surface tension, was derived from potential flow equation. The results show that, when forced frequency is lower, the effect of surface tension on mode selection of surface wave is not important. However, when forced frequency is higher, the surface tension can not be neglected. This proved that the surface tension causes free surface returning to equilibrium location. In addition, due to considering the effect of surface tension, the theoretical result approaches to experimental results much more than that of no surface tension.

  20. Spin-split bands of metallic hydrogenated ZnO ( 10 1 ¯ 0 surface: First-principles study

    Directory of Open Access Journals (Sweden)

    Moh. Adhib Ulil Absor

    2016-02-01

    Full Text Available For spintronics applications, generation of significant spin transport is required, which is achieved by applying a semiconductor surface exhibiting metallic spin-split surface-state bands. We show that metallic spin-split surface-state bands are achieved on hydrogenated ZnO ( 10 1 ¯ 0 surface by using first-principles density-functional theory calculations. We find that these metallic surface-state bands with dominant Zn-s and p orbitals exhibit Rashba spin splitting with a strong anisotropic character. This finding makes spintronics devices using oxide electronics surface materials possible.

  1. Reduced dimensionality spin-orbit dynamics of CH3 + HCl ⇌ CH4 + Cl on ab initio surfaces.

    Science.gov (United States)

    Remmert, Sarah M; Banks, Simon T; Harvey, Jeremy N; Orr-Ewing, Andrew J; Clary, David C

    2011-05-28

    A reduced dimensionality quantum scattering method is extended to the study of spin-orbit nonadiabatic transitions in the CH(3) + HCl ⇌ CH(4) + Cl((2)P(J)) reaction. Three two-dimensional potential energy surfaces are developed by fitting a 29 parameter double-Morse function to CCSD(T)/IB//MP2/cc-pV(T+d)Z-dk ab initio data; interaction between surfaces is described by geometry-dependent spin-orbit coupling functions fit to MCSCF/cc-pV(T+d)Z-dk ab initio data. Spectator modes are treated adiabatically via inclusion of curvilinear projected frequencies. The total scattering wave function is expanded in a vibronic basis set and close-coupled equations are solved via R-matrix propagation. Ground state thermal rate constants for forward and reverse reactions agree well with experiment. Multi-surface reaction probabilities, integral cross sections, and initial-state selected branching ratios all highlight the importance of vibrational energy in mediating nonadiabatic transition. Electronically excited state dynamics are seen to play a small but significant role as consistent with experimental conclusions.

  2. Spin excitations in 3D molecular magnets probed by neutron scattering

    CERN Document Server

    Bordallo, H N; Chapon, L C; Manson, J L; Cook, J C; Lee, S H; Copley, J R D; Yildirim, T; Kern, S

    2002-01-01

    The emerging field of molecular magnetism constitutes a new branch of materials science that deals with the magnetic properties of molecules, or assemblies of molecules, that contain magnetic centers. The growing interest in understanding the origin of the magnetic ordering in these materials is to obtain novel multiproperty molecular magnetic materials with high transition temperatures. Molecules based on the dicyanamide ion [N ident to C-N-C ident to N], abbreviated (dca), such as M(dca) sub 2 [M=Mn, Ni], have shown interesting bulk properties that prompted our inelastic neutron scattering (INS) studies. While the Mn sup 2 sup + ion is isotropic because of its L=0 configuration, the isostructural Ni analog has S=1 and demonstrates marked single-ion anisotropy. Mn(dca) sub 2 is a canted antiferromagnet below 16 K, while Ni(dca) sub 2 is a ferromagnet below 21 K. INS has been used to investigate the magnetic excitations in Mn(dca) sub 2 and Ni(dca) sub 2. For Mn(dca) sub 2 , a Heisenberg model gives good corr...

  3. Hot electron mediated desorption rates calculated from excited state potential energy surfaces

    CERN Document Server

    Olsen, Thomas; Schiøtz, Jakob

    2008-01-01

    We present a model for Desorption Induce by (Multiple) Electronic Transitions (DIET/DIMET) based on potential energy surfaces calculated with the Delta Self-Consistent Field extension of Density Functional Theory. We calculate potential energy surfaces of CO and NO molecules adsorbed on various transition metal surfaces, and show that classical nuclear dynamics does not suffice for propagation in the excited state. We present a simple Hamiltonian describing the system, with parameters obtained from the excited state potential energy surface, and show that this model can describe desorption dynamics in both the DIET and DIMET regime, and reproduce the power law behavior observed experimentally. We observe that the internal stretch degree of freedom in the molecules is crucial for the energy transfer between the hot electrons and the molecule when the coupling to the surface is strong.

  4. Glass-like recovery of antiferromagnetic spin ordering in a photo-excited manganite Pr0.7Ca0.3MnO3

    Energy Technology Data Exchange (ETDEWEB)

    Zhou, S. Y.; Langner, M. C.; Zhu, Y.; Chuang, Y. -D.; Rini, M.; Glover, T. E.; Hertlein, M. P.; Gonzalez, A.G. Cruz; Tahir, N.; Tomioka, Y.; Tokura, Y.; Hussain, Z.; Schoenlein, R. W.

    2014-01-16

    Electronic orderings of charges, orbitals and spins are observed in many strongly correlated electron materials, and revealing their dynamics is a critical step toward understanding the underlying physics of important emergent phenomena. Here we use time-resolved resonant soft x-ray scattering spectroscopy to probe the dynamics of antiferromagnetic spin ordering in the manganite Pr0:7Ca0:3MnO3 following ultrafast photo-exitation. Our studies reveal a glass-like recovery of the spin ordering and a crossover in the dimensionality of the restoring interaction from quasi-1D at low pump fluence to 3D at high pump fluence. This behavior arises from the metastable state created by photo-excitation, a state characterized by spin disordered metallic droplets within the larger charge- and spin-ordered insulating domains. Comparison with time-resolved resistivity measurements suggests that the collapse of spin ordering is correlated with the insulator-to-metal transition, but the recovery of the insulating phase does not depend on the re-establishment of the spin ordering.

  5. Excitation of the Uller-Zenneck electromagnetic surface waves in the prism-coupled configuration

    Science.gov (United States)

    Rasheed, Mehran; Faryad, Muhammad

    2017-08-01

    A configuration to excite the Uller-Zenneck surface electromagnetic waves at the planar interfaces of homogeneous and isotropic dielectric materials is proposed and theoretically analyzed. The Uller-Zenneck waves are surface waves that can exist at the planar interface of two dissimilar dielectric materials of which at least one is a lossy dielectric material. In this paper, a slab of a lossy dielectric material was taken with lossless dielectric materials on both sides. A canonical boundary-value problem was set up and solved to find the possible Uller-Zenneck waves and waveguide modes. The Uller-Zenneck waves guided by the slab of the lossy dielectric material were found to be either symmetric or antisymmetric and transmuted into waveguide modes when the thickness of that slab was increased. A prism-coupled configuration was then successfully devised to excite the Uller-Zenneck waves. The results showed that the Uller-Zenneck waves are excited at the same angle of incidence for any thickness of the slab of the lossy dielectric material, whereas the waveguide modes can be excited when the slab is sufficiently thick. The excitation of Uller-Zenneck waves at the planar interfaces with homogeneous and all-dielectric materials can usher in new avenues for the applications for electromagnetic surface waves.

  6. Quantum model of a solid-state spin qubit: Ni cluster on a silicon surface by the generalized spin Hamiltonian and X-ray absorption spectroscopy investigations

    Science.gov (United States)

    Farberovich, Oleg V.; Mazalova, Victoria L.; Soldatov, Alexander V.

    2015-11-01

    We present here the quantum model of a Ni solid-state electron spin qubit on a silicon surface with the use of a density-functional scheme for the calculation of the exchange integrals in the non-collinear spin configurations in the generalized spin Hamiltonian (GSH) with the anisotropic exchange coupling parameters linking the nickel ions with a silicon substrate. In this model the interaction of a spin qubit with substrate is considered in GSH at the calculation of exchange integrals Jij of the nanosystem Ni7-Si in the one-electron approach taking into account chemical bonds of all Si-atoms of a substrate (environment) with atoms of the Ni7-cluster. The energy pattern was found from the effective GSH Hamiltonian acting in the restricted spin space of the Ni ions by the application of the irreducible tensor operators (ITO) technique. In this paper we offer the model of the quantum solid-state N-spin qubit based on the studying of the spin structure and the spin-dynamics simulations of the 3d-metal Ni clusters on the silicon surface. The solution of the problem of the entanglement between spin states in the N-spin systems is becoming more interesting when considering clusters or molecules with a spectral gap in their density of states. For quantifying the distribution of the entanglement between the individual spin eigenvalues (modes) in the spin structure of the N-spin system we use the density of entanglement (DOE). In this study we have developed and used the advanced high-precision numerical techniques to accurately assess the details of the decoherence process governing the dynamics of the N-spin qubits interacting with a silicon surface. We have studied the Rabi oscillations to evaluate the N-spin qubits system as a function of the time and the magnetic field. We have observed the stabilized Rabi oscillations and have stabilized the quantum dynamical qubit state and Rabi driving after a fixed time (0.327 μs). The comparison of the energy pattern with the

  7. Equation-of-Motion Coupled-Cluster Theory for Excitation Energies of Closed-Shell Systems with Spin-Orbit Coupling.

    Science.gov (United States)

    Wang, Zhifan; Tu, Zheyan; Wang, Fan

    2014-12-09

    Excitation energies of closed-shell systems based on the equation-of-motion (EOM) coupled-cluster theory at the singles and doubles (CCSD) level with spin-orbit coupling (SOC) included in the post-Hartree-Fock treatment are implemented in the present work. SOC can be included in both the CC and EOM steps (EOM-SOC-CCSD) or only in the EOM part (SOC-EOM-CCSD). The latter approach is an economical way to account for SOC effects, but excitation energies with this approach are not size-intensive. When the unlinked term in the latter approach is neglected (cSOC-EOM-CCSD), size-intensive excitation energies can be obtained. Time-reversal symmetry and spatial symmetry are exploited to reduce the computational effort. Imposing time-reversal symmetry results in a real matrix representation for the similarity-transformed Hamiltonian, which facilitates the requirement of time-reversal symmetry for new trial vectors in Davidson's algorithm. Results on some closed-shell atoms and molecules containing heavy elements show that EOM-SOC-CCSD can provide excitation energies and spin-orbit splittings with reasonable accuracy. On the other hand, the SOC-EOM-CCSD approach is able to afford accurate estimates of SOC effects for valence electrons of systems containing elements up to the fifth row, while cSOC-EOM-CCSD is less accurate for spin-orbit splittings of transitions involving p1/2 spinors, even for Kr.

  8. Quantum dynamics of excitations and decoherence in many-spin systems detected with Loschmidt echoes: its relation to their spreading through the Hilbert space.

    Science.gov (United States)

    Sánchez, C M; Levstein, P R; Buljubasich, L; Pastawski, H M; Chattah, A K

    2016-06-13

    In this work, we overview time-reversal nuclear magnetic resonance (NMR) experiments in many-spin systems evolving under the dipolar Hamiltonian. The Loschmidt echo (LE) in NMR is the signal of excitations which, after evolving with a forward Hamiltonian, is recovered by means of a backward evolution. The presence of non-diagonal terms in the non-equilibrium density matrix of the many-body state is directly monitored experimentally by encoding the multiple quantum coherences. This enables a spin counting procedure, giving information on the spreading of an excitation through the Hilbert space and the formation of clusters of correlated spins. Two samples representing different spin systems with coupled networks were used in the experiments. Protons in polycrystalline ferrocene correspond to an 'infinite' network. By contrast, the liquid crystal N-(4-methoxybenzylidene)-4-butylaniline in the nematic mesophase represents a finite proton system with a hierarchical set of couplings. A close connection was established between the LE decay and the spin counting measurements, confirming the hypothesis that the complexity of the system is driven by the coherent dynamics.

  9. Robust and thermal-healing superhydrophobic surfaces by spin-coating of polydimethylsiloxane.

    Science.gov (United States)

    Long, Mengying; Peng, Shan; Deng, Wanshun; Yang, Xiaojun; Miao, Kai; Wen, Ni; Miao, Xinrui; Deng, Wenli

    2017-12-15

    Superhydrophobic surfaces easily lose their excellent water-repellency after damages, which limit their broad applications in practice. Thus, the fabrication of superhydrophobic surfaces with excellent durability and thermal healing should be taken into consideration. In this work, robust superhydrophobic surfaces with thermal healing were successfully fabricated by spin-coating method. To achieve superhydrophobicity, cost-less and fluoride-free polydimethylsiloxane (PDMS) was spin-coated on rough aluminum substrates. After being spin-coated for one cycle, the superhydrophobic PDMS coated hierarchical aluminum (PDMS-H-Al) surfaces showed excellent tolerance to various chemical and mechanical damages in lab, and outdoor damages for 90days. When the PDMS-H-Al surfaces underwent severe damages such as oil contamination (peanut oil with high boiling point) or sandpaper abrasion (500g of force for 60cm), their superhydrophobicity would lose. Interestingly, through a heating process, cyclic oligomers generating from the partially decomposed PDMS acted as low-surface-energy substance on the damaged rough surfaces, leading to the recovery of superhydrophobicity. The relationship between the spin-coating cycles and surface wettability was also investigated. This paper provides a facile, fluoride-free and efficient method to fabricate superhydrophobic surfaces with thermal healing. Copyright © 2017. Published by Elsevier Inc.

  10. Control of light polarization using optically spin-injected vertical external cavity surface emitting lasers

    Energy Technology Data Exchange (ETDEWEB)

    Frougier, J., E-mail: julien.frougier@thalesgroup.com; Jaffrès, H.; Deranlot, C.; George, J.-M. [Unité Mixte de Physique CNRS-Thales and Université Paris Sud 11, 1 av. Fresnel, 91767 Palaiseau (France); Baili, G.; Dolfi, D. [Thales Research and Technology, 1 av. Fresnel, 91767 Palaiseau (France); Alouini, M. [Institut de Physique de Rennes, 263 Avenue Général Leclerc, 35042 Rennes (France); Sagnes, I. [Laboratoire de Photonique et de Nanostructures, Route de Nozay, 91460 Marcoussis (France); Garnache, A. [Institut d' électronique du Sud CNRS UMR5214, Université Montpellier 2 Place Eugene Bataillon, 34095 Montpellier (France)

    2013-12-16

    We fabricated and characterized an optically pumped (100)-oriented InGaAs/GaAsP multiple quantum well Vertical External Cavity Surface Emitting Laser (VECSEL). The structure is designed to allow the integration of a Metal-Tunnel-Junction ferromagnetic spin-injector for future electrical injection. We report here the control at room temperature of the electromagnetic field polarization using optical spin injection in the active medium of the VECSEL. The switching between two highly circular polarization states had been demonstrated using an M-shaped extended cavity in multi-modes lasing. This result witnesses an efficient spin-injection in the active medium of the LASER.

  11. Spin Polarization Inversion at Benzene-Absorbed Fe4N Surface

    KAUST Repository

    Zhang, Qian

    2015-05-27

    We report a first-principle study on electronic structure and simulation of the spin-polarized scanning tunneling microscopy graphic of a benzene/Fe4N interface. Fe4N is a compound ferromagnet suitable for many spintronic applications. We found that, depending on the particular termination schemes and interface configurations, the spin polarization on the benzene surface shows a rich variety of properties ranging from cosine-type oscillation to polarization inversion. Spin-polarization inversion above benzene is resulting from the hybridizations between C pz and the out-of-plane d orbitals of Fe atom.

  12. The role of core excitations in the structure and decay of the 16+ spin-gap isomer in 96Cd

    Directory of Open Access Journals (Sweden)

    P.J. Davies

    2017-04-01

    Full Text Available The first evidence for β-delayed proton emission from the 16+ spin gap isomer in 96Cd is presented. The data were obtained from the Rare Isotope Beam Factory, at the RIKEN Nishina Center, using the BigRIPS spectrometer and the EURICA decay station. βp branching ratios for the ground state and 16+ isomer have been extracted along with more precise lifetimes for these states and the lifetime for the ground state decay of 95Cd. Large scale shell model (LSSM calculations have been performed and WKB estimates made for ℓ=0,2,4 proton emission from three resonance-like states in 96Ag, that are populated by the β decay of the isomer, and the results compared to the new data. The calculations suggest that ℓ=2 proton emission from the resonance states, which reside ∼5 MeV above the proton separation energy, dominates the proton decay. The results highlight the importance of core-excited wavefunction components for the 16+ state.

  13. Dynamics of an unbalanced ring spinning on a rough horizontal surface

    OpenAIRE

    Budiman, Benny S.

    1993-01-01

    An interesting stability property, as fascinating as that of spinning tops and gyroscopes, is observable in the motion of an unbalanced ring spinning on a rough horizontal surface. An analytical and numerical study is performed to investigate the general motion of an unbalanced ring modeled as a thin ring with a particle attached to its rim. The translational motion is represented by the rectangular coordinates of the ring geometric center. The rotational motion is represented by a 1-2-3 set ...

  14. Potential energy surfaces and approximate kinetic model for the excited state dynamics of Pigment Yellow 101

    NARCIS (Netherlands)

    Fletcher, Katharyn; Dreuw, Andreas; Faraji, Shirin

    2014-01-01

    Pigment Yellow 101 (PY101) exhibits a rich photochemistry in its S-1 state as it undergoes excited state intramolecular proton transfer and trans-cis isomerizations upon photoexcitation. Relaxed scans of its potential energy surface are thus computed along the reaction paths connecting the six most

  15. Elliptically polarized modes for the unidirectional excitation of surface plasmon polaritons

    NARCIS (Netherlands)

    Compaijen, Paul J.; Malyshev, Victor A.; Knoester, Jasper

    2016-01-01

    We propose a new method for the directional excitation of surface plasmon polaritons by a metal nanoparticle antenna, based on the elliptical polarization of the normal modes of the antenna when it is in close proximity to a metallic substrate. The proposed theoretical model allows for the full char

  16. Topology optimization of grating couplers for the efficient excitation of surface plasmons

    DEFF Research Database (Denmark)

    Andkjær, Jacob Anders; Sigmund, Ole; Nishiwaki, Shinji

    2010-01-01

    We propose a methodology for a systematic design of grating couplers for efficient excitation of surface plasmons at metal-dielectric interfaces. The methodology is based on a two-dimensional topology optimization formulation based on the H-polarized scalar Helmholtz equation and finite-element m...

  17. Application of a grating coupler for surface plasmon polariton excitation in a photoemission electron microscopy experiment

    DEFF Research Database (Denmark)

    Leißner, Till; Jauernik, Stephan; Lemke, Christoph

    Surface plasmon polariton (SPP) excitation at a gold-vacuum interface via 800 nm light pulses mediated by a periodic array of gold ridges is probed at high lateral resolution by means of photoemission electron microscopy (PEEM). We directly monitor and quantify the coupling properties as a function...

  18. Giant enhancement of sum-frequency yield by surface-plasmon excitation

    NARCIS (Netherlands)

    van der Ham, E. W. M.; Vrehen, Q. H. F.; Eliel, E. R.; Yakovlev, V. A.; Valieva, E. V.; Kuzik, L. A.; Petrov, J. E.; Sychugov, V. A.; van der Meer, A. F. G.

    1999-01-01

    We show experimentally that the radiation generated in infrared-visible sum-frequency mixing at an air-silver interface can be greatly enhanced when the visible input beam excites a surface plasmon-polariton at the interface. With either a prism or a grating used to couple the visible radiation with

  19. Ultrahigh Enhancement of Electromagnetic Fields by Exciting Localized with Extended Surface Plasmons

    CERN Document Server

    Li, Anran; Abdulhalim, Ibrahim; Li, Shuzhou

    2015-01-01

    Excitation of localized surface plasmons (LSPs) of metal nanoparticles (NPs) residing on a flat metal film has attracted great attentions recently due to the enhanced electromagnetic (EM) fields found to be higher than the case of NPs on a dielectric substrate. In the present work, it is shown that even much higher enhancement of EM fields is obtained by exciting the LSPs through extended surface plasmons (ESPs) generated at the metallic film surface using the Kretschmann-Raether configuration. We show that the largest EM field enhancement and the highest surface-enhanced fluorescence intensity are obtained when the incidence angle is the ESP resonance angle of the underlying metal film. The finite-difference time-domain simulations indicate that excitation of LSPs using ESPs can generate 1-3 orders higher EM field intensity than direct excitation of the LSPs using incidence from free space. The ultrahigh enhancement is attributed to the strong confinement of the ESP waves in the vertical direction. The drast...

  20. Theoretical and experimental study of the vibrational excitations in ethane monolayers adsorbed on graphite (0001) surfaces

    DEFF Research Database (Denmark)

    Hansen, Flemming Yssing; Taub, H.

    1987-01-01

    The collective vibrational excitations of two different crystalline monolayer phases of ethane (C2H6) adsorbed on the graphite (0001) surface have been investigated theoretically and experimentally. The monolayer phases studied are the commensurate 7/8 ×4 structure in which the ethane molecules lie...

  1. Modeling the collective excitations in a full Heusler Co{sub 2} FeAl{sub 0.5} Si{sub 0.5} (CFAS) spin valve magnetic nanopillar in the electromagnetic field

    Energy Technology Data Exchange (ETDEWEB)

    David, Cherine; Arumugam, Brinda; Rajamani, Amuda, E-mail: amuvenkat@gmail.com; Natarajan, Kanimozhi

    2014-12-15

    This paper describes the physics of collective excitations that are caused by spin-transfer torques in CFAS magnetic multilayer. When the magnetizations of the pinned and free layers are not collinear with each other, the spin-polarized currents transfer angular momentum to the magnetizations near the interfaces, giving rise to spin-transfer torques. The currents in magnetic multilayer are spin polarised and can carry enough angular momentum. When an electron spin carried by the current interacts with a magnetic layer, the exchange interaction leads to torque between the spin and the magnetization vector of the free layer. This is Spin Transfer Torque (STT) and it excites the magnetization when it is large enough. The Spin Transfer Torque induced collective excitations for the CFAS spin valve pillar have been extensively studied in this paper. - Highlights: • We have modeled LLGS equation for CFAS multilayer array. • The dynamics of collective excitation induced by STT is investigated. • The interactions exhibit solitonic behaviour at both limiting modes of polarization. • The spin components of the solitons are graphically represented.

  2. Excitation of unsteady Görtler vortices by localized surface nonuniformities

    Science.gov (United States)

    Boiko, A. V.; Ivanov, A. V.; Kachanov, Yu. S.; Mischenko, D. A.; Nechepurenko, Yu. M.

    2016-08-01

    A combined theoretical and numerical analysis of an experiment devoted to the excitation of Görtler vortices by localized stationary or vibrating surface nonuniformities in a boundary layer over a concave surface is performed. A numerical model of generation of small-amplitude disturbances and their downstream propagation based on parabolic equations is developed. In the framework of this model, the optimal and the modal parts of excited disturbance are defined as solutions of initial-value problems with initial values being, respectively, the optimal disturbance and the leading local mode at the location of the source. It is shown that a representation of excited disturbance as a sum of the optimal part and a remainder makes it possible to describe its generation and downstream propagation, as well as to predict satisfactorily the corresponding receptivity coefficient. In contrast, the representation based on the modal part provides only coarse information about excitation and propagation of disturbance in the range of parameters under investigation. However, it is found that the receptivity coefficients estimated using the modal parts can be reinterpreted to preserve their practical significance. A corresponding procedure was developed. The theoretical and experimental receptivity coefficients are estimated and compared. It is found that the receptivity magnitudes grow significantly with the disturbance frequency. Variation of the span-wise scale of the nonuniformities affects weakly the receptivity characteristics at zero frequency. However, at high frequencies, the efficiency of excitation of Görtler vortices depends substantially on the span-wise scale.

  3. Excitation of unsteady Görtler vortices by localized surface nonuniformities

    Science.gov (United States)

    Boiko, A. V.; Ivanov, A. V.; Kachanov, Yu. S.; Mischenko, D. A.; Nechepurenko, Yu. M.

    2017-02-01

    A combined theoretical and numerical analysis of an experiment devoted to the excitation of Görtler vortices by localized stationary or vibrating surface nonuniformities in a boundary layer over a concave surface is performed. A numerical model of generation of small-amplitude disturbances and their downstream propagation based on parabolic equations is developed. In the framework of this model, the optimal and the modal parts of excited disturbance are defined as solutions of initial-value problems with initial values being, respectively, the optimal disturbance and the leading local mode at the location of the source. It is shown that a representation of excited disturbance as a sum of the optimal part and a remainder makes it possible to describe its generation and downstream propagation, as well as to predict satisfactorily the corresponding receptivity coefficient. In contrast, the representation based on the modal part provides only coarse information about excitation and propagation of disturbance in the range of parameters under investigation. However, it is found that the receptivity coefficients estimated using the modal parts can be reinterpreted to preserve their practical significance. A corresponding procedure was developed. The theoretical and experimental receptivity coefficients are estimated and compared. It is found that the receptivity magnitudes grow significantly with the disturbance frequency. Variation of the span-wise scale of the nonuniformities affects weakly the receptivity characteristics at zero frequency. However, at high frequencies, the efficiency of excitation of Görtler vortices depends substantially on the span-wise scale.

  4. Surface Landau levels and spin states in bismuth (111) ultrathin films.

    Science.gov (United States)

    Du, Hongjian; Sun, Xia; Liu, Xiaogang; Wu, Xiaojun; Wang, Jufeng; Tian, Mingyang; Zhao, Aidi; Luo, Yi; Yang, Jinlong; Wang, Bing; Hou, J G

    2016-03-11

    The development of next-generation electronics is much dependent on the discovery of materials with exceptional surface-state spin and valley properties. Because of that, bismuth has attracted a renewed interest in recent years. However, despite extensive studies, the intrinsic electronic transport properties of Bi surfaces are largely undetermined due to the strong interference from the bulk. Here we report the unambiguous determination of the surface-state Landau levels in Bi (111) ultrathin films using scanning tunnelling microscopy under magnetic fields perpendicular to the surface. The Landau levels of the electron-like and the hole-like carriers are accurately characterized and well described by the band structure of the Bi (111) surface from density functional theory calculations. Some specific surface spin states with a large g-factor are identified. Our findings shed light on the exploiting surface-state properties of Bi for their applications in spintronics and valleytronics.

  5. Spin wave surface states in one-dimensional planar magnonic crystals

    CERN Document Server

    Rychły, Justyna

    2016-01-01

    We have investigated surface spin wave states in one-dimensional planar bi-component magnonic crystals, localized on the surfaces resulting from the breaking of the periodic structure. The two systems have been considered: the magnonic crystal with periodic changes of the anisotropy field in exchange regime and the magnonic crystal composed of Fe and Ni stripes in dipolar regime with exchange interactions included. We chose the symmetric unit cell for both systems to implement the symmetry related criteria for existence of the surface states. We investigated also the surface states induced by the presence of perturbation of the surface areas of the magnonic crystals. We showed, that the system with modulated anisotropy is a direct analog of the electronic crystal. Therefore, the surface states in both systems have the same properties. For surface states existing in magnonic crystals in dipolar regime we demonstrated that spin waves preserve distinct differences to the electronic crystals, which are due to lon...

  6. Pseudo-Spin Model for the Cytoskeletal Microtubule Surface

    Institute of Scientific and Technical Information of China (English)

    CHEN Ying; QIU Xi-Jun; LI Ru-Xin

    2004-01-01

    @@ Due to the inherent symmetry structures and the electric properties in the microtubule (MT), we treat the MT as a one-dimensional ferroelectric system and describe the nonlinear dynamics of dimer electric dipoles in one protofilament of the MT by virtue of the double-well potential. Consequently, the physical problem has been mapped onto the pseudo-spin system, and the mean-field approximation has been taken to obtain some physical results, including the expression for the phase transition temperature Tc and the estimated value of Tc (≈ 312 K).

  7. Optically excited structural transition in atomic wires on surfaces at the quantum limit

    Science.gov (United States)

    Frigge, T.; Hafke, B.; Witte, T.; Krenzer, B.; Streubühr, C.; Samad Syed, A.; Mikšić Trontl, V.; Avigo, I.; Zhou, P.; Ligges, M.; von der Linde, D.; Bovensiepen, U.; Horn-von Hoegen, M.; Wippermann, S.; Lücke, A.; Sanna, S.; Gerstmann, U.; Schmidt, W. G.

    2017-03-01

    Transient control over the atomic potential-energy landscapes of solids could lead to new states of matter and to quantum control of nuclear motion on the timescale of lattice vibrations. Recently developed ultrafast time-resolved diffraction techniques combine ultrafast temporal manipulation with atomic-scale spatial resolution and femtosecond temporal resolution. These advances have enabled investigations of photo-induced structural changes in bulk solids that often occur on timescales as short as a few hundred femtoseconds. In contrast, experiments at surfaces and on single atomic layers such as graphene report timescales of structural changes that are orders of magnitude longer. This raises the question of whether the structural response of low-dimensional materials to femtosecond laser excitation is, in general, limited. Here we show that a photo-induced transition from the low- to high-symmetry state of a charge density wave in atomic indium (In) wires supported by a silicon (Si) surface takes place within 350 femtoseconds. The optical excitation breaks and creates In-In bonds, leading to the non-thermal excitation of soft phonon modes, and drives the structural transition in the limit of critically damped nuclear motion through coupling of these soft phonon modes to a manifold of surface and interface phonons that arise from the symmetry breaking at the silicon surface. This finding demonstrates that carefully tuned electronic excitations can create non-equilibrium potential energy surfaces that drive structural dynamics at interfaces in the quantum limit (that is, in a regime in which the nuclear motion is directed and deterministic). This technique could potentially be used to tune the dynamic response of a solid to optical excitation, and has widespread potential application, for example in ultrafast detectors.

  8. Optically excited structural transition in atomic wires on surfaces at the quantum limit.

    Science.gov (United States)

    Frigge, T; Hafke, B; Witte, T; Krenzer, B; Streubühr, C; Samad Syed, A; Mikšić Trontl, V; Avigo, I; Zhou, P; Ligges, M; von der Linde, D; Bovensiepen, U; Horn-von Hoegen, M; Wippermann, S; Lücke, A; Sanna, S; Gerstmann, U; Schmidt, W G

    2017-03-29

    Transient control over the atomic potential-energy landscapes of solids could lead to new states of matter and to quantum control of nuclear motion on the timescale of lattice vibrations. Recently developed ultrafast time-resolved diffraction techniques combine ultrafast temporal manipulation with atomic-scale spatial resolution and femtosecond temporal resolution. These advances have enabled investigations of photo-induced structural changes in bulk solids that often occur on timescales as short as a few hundred femtoseconds. In contrast, experiments at surfaces and on single atomic layers such as graphene report timescales of structural changes that are orders of magnitude longer. This raises the question of whether the structural response of low-dimensional materials to femtosecond laser excitation is, in general, limited. Here we show that a photo-induced transition from the low- to high-symmetry state of a charge density wave in atomic indium (In) wires supported by a silicon (Si) surface takes place within 350 femtoseconds. The optical excitation breaks and creates In-In bonds, leading to the non-thermal excitation of soft phonon modes, and drives the structural transition in the limit of critically damped nuclear motion through coupling of these soft phonon modes to a manifold of surface and interface phonons that arise from the symmetry breaking at the silicon surface. This finding demonstrates that carefully tuned electronic excitations can create non-equilibrium potential energy surfaces that drive structural dynamics at interfaces in the quantum limit (that is, in a regime in which the nuclear motion is directed and deterministic). This technique could potentially be used to tune the dynamic response of a solid to optical excitation, and has widespread potential application, for example in ultrafast detectors.

  9. Highly Efficient Excitation of Surface Plasmons Using a Si Gable Tip

    CERN Document Server

    Dewanjee, Arnab; Aitchison, J Stewart; Mojahedi, Mo

    2016-01-01

    We propose a novel technique to efficiently excite a surface plasmon polariton (SPP) mode at a gold-glass interface by using an engineered high index (silicon) gabled tip at the telecom wavelengths. The proposed structure can theoretically convert 49% of the input optical power to a SPP mode. Also we experimentally validate the effective high efficiency coupling by the gabled tip. The device is compact, it will facilitate the on-chip excitation of the SPP, its fabrication is compatible with the standard Si fabrication processes, and as such, it is expected to be useful in the design of future integrated sensors.

  10. Casimir-Polder forces in the presence of thermally excited surface modes

    CERN Document Server

    Laliotis, Athanasios; Maurin, Isabelle; Ducloy, Martial; Bloch, Daniel

    2014-01-01

    The temperature dependence of the Casimir-Polder interaction addresses fundamental issues for understanding vacuum and thermal fluctuations. It is highly sensitive to surface waves which, in the near field, govern the thermal emission of a hot surface. Here we use optical reflection spectroscopy to monitor the atom-surface interaction between a Cs*(7D3/2) atom and a hot sapphire surface at a distance ~ 100 nm. In our experiments, that explore a large range of temperatures (500-1000K) the hot surface is at thermal equilibrium with the vacuum. The observed increase of the interaction with temperature, by up to 50 %, relies on the coupling between atomic virtual transitions in the infrared range and thermally excited surface-polariton modes. We extrapolate our findings to a broad distance range, from the isolated free atom to the short distances relevant to physical chemistry. Our work also opens the prospect of controlling atom surface interactions by engineering thermal fields.

  11. Stability and bifurcation analysis of spin-polarized vertical-cavity surface-emitting lasers

    Science.gov (United States)

    Li, Nianqiang; Susanto, H.; Cemlyn, B. R.; Henning, I. D.; Adams, M. J.

    2017-07-01

    A detailed stability and bifurcation analysis of spin-polarized vertical-cavity surface-emitting lasers (VCSELs) is presented. We consider both steady-state and dynamical regimes. In the case of steady-state operation, we carry out a small-signal (asymptotic) stability analysis of the steady-state solutions for a representative set of spin-VCSEL parameters. Compared with full numerical simulation, we show this produces surprisingly accurate results over the whole range of pump ellipticity, and spin-VCSEL bias up to 1.5 times the threshold. We then combine direct numerical integration of the extended spin-flip model and standard continuation technique to examine the underlying dynamics. We find that the spin VCSEL undergoes a period-doubling or quasiperiodic route to chaos as either the pump magnitude or polarization ellipticity is varied. Moreover, we find that different dynamical states can coexist in a finite interval of pump intensity, and observe a hysteresis loop whose width is tunable via the pump polarization. Finally we report a comparison of stability maps in the plane of the pump polarization against pump magnitude produced by categorizing the dynamic output of a spin VCSEL from time-domain simulations, against supercritical bifurcation curves obtained by the standard continuation package auto. This helps us better understand the underlying dynamics of the spin VCSELs.

  12. Surface atmospheric pressure excitation of the translational mode of the inner core

    CERN Document Server

    Rosat, Séverine; Rogister, Yves

    2014-01-01

    Using hourly atmospheric surface pressure field from ECMWF (European Centre for Medium-Range Weather Forecasts) and from NCEP (National Centers for Environmental Prediction) Climate Forecast System Reanalysis (CFSR) models, we show that atmospheric pressure fluctuations excite the translational oscillation of the inner core, the so-called Slichter mode, to the sub-nanogal level at the Earth surface. The computation is performed using a normal-mode formalism for a spherical, self-gravitating anelastic PREM-like Earth model. We determine the statistical response in the form of power spectral densities of the degree-one spherical harmonic components of the observed pressure field. Both hypotheses of inverted and non-inverted barometer for the ocean response to pressure forcing are considered. Based on previously computed noise levels, we show that the surface excitation amplitude is below the limit of detection of the superconducting gravimeters, making the Slichter mode detection a challenging instrumental task...

  13. Excitation of surface and volume plasmons in metal nanocluster by fast electrons

    CERN Document Server

    Gildenburg, V B; Pavlichenko, I A

    2015-01-01

    Surface and volume plasmons excited in a metal cluster by moving electron and corresponding inelastic scattering spectra are studied based on the hydrodynamic approach. Along with the bulk losses traditionally taken into account, the surface and radiative ones are also considered as the physical mechanisms responsible for the plasmon damping. The second and third mechanisms are found to be essential for the surface plasmons and depend very differently on the multipole mode order. The differential equations are obtained which describe the temporal evolution of every particular mode as that one of a linear oscillator excited by the given external force, and the electron energy loss spectra are calculated. The changes in spectrum shape with the impact parameter and with the electron passage time are analyzed and found to be in good enough agreement with the data of scanning transmission electron microscopy (STEM) experiments. It is shown that, in the general case, a pronounced contribution to the formation of th...

  14. Excitation and propagation of shear-horizontal-type surface and bulk acoustic waves.

    Science.gov (United States)

    Hashimoto, K Y; Yamaguchi, M

    2001-09-01

    This paper reviews the basic properties of shear-horizontal (SH)-type surface acoustic waves (SAWs) and bulk acoustic waves (BAWs). As one of the simplest cases, the structure supporting Bleustein-Gulyaev-Shimizu waves is considered, and their excitation and propagation are discussed from various view points. First, the formalism based on the complex integral theory is presented, where the surface is assumed to be covered with an infinitesimally thin metallic film, and it is shown how the excitation and propagation of SH-type waves are affected by the surface perturbation. Then, the analysis is extended to a periodic grating structure, and the behavior of SH-type SAWs under the grating structure is discussed. Finally, the origin of the leaky nature is explained.

  15. Spin excitations in a K0.84Fe1.99Se2 superconductor as studied by M(o)ssbauer spectroscopy

    Institute of Scientific and Technical Information of China (English)

    Li Zhi-Wei; Ma Xiao-Ming; Pang Hua; Li Fa-Shen

    2012-01-01

    M(o)ssbauer spectroscopy was used to probe the site-specific information of a K0.84Fe1.99Se2 superconductor.A spin excitation gap,△E ≈ 5.5 meV,is observed by analyzing the temperature dependence of the hyperfine magnetic field (HMF) at the iron site within the spin wave theory. Using the simple model suggested in the literature,the temperature dependence of the HMF is well reproduced,suggesting that,below room temperature,the alkali metal intercalated iron-selenide superconductors can be regarded as ferromagnetically coupled spin blocks that interact with each other antiferromagnetically to form the observed checkerboard-like magnetic structure.

  16. Ultrafast circular polarization oscillations in spin-polarized vertical-cavity surface-emitting laser devices

    Science.gov (United States)

    Gerhardt, N. C.; Li, M.; Jaehme, H.; Soldat, H.; Hofmann, M. R.; Ackemann, T.

    2010-02-01

    Spin-polarized lasers offer new encouraging possibilities for future devices. We investigate the polarization dynamics of electrically pumped vertical-cavity surface-emitting lasers after additional spin injection at room temperature. We find that the circular polarization degree exhibits faster dynamics than the emitted light. Moreover the experimental results demonstrate a strongly damped ultrafast circular polarization oscillation due to spin injection with an oscillation frequency of approximately 11GHz depending on the birefringence in the VCSEL device. We compare our experimental results with theoretical calculations based on rate-equations. This allows us to predict undamped long persisting ultrafast polarization oscillations, which reveal the potential of spin-VCSELs for ultrafast modulation applications.

  17. Strong spin-orbit interaction of light on the surface of atomically thin crystals

    Science.gov (United States)

    Liu, Mengxia; Cai, Liang; Chen, Shizhen; Liu, Yachao; Luo, Hailu; Wen, Shuangchun

    2017-06-01

    The photonic spin Hall effect (SHE) can be regarded as a direct optical analogy of the SHE in electronic systems where a refractive index gradient plays the role of an electric potential. However, it has been demonstrated that the effective refractive index fails to adequately explain the light-matter interaction in atomically thin crystals. In this paper, we examine the spin-orbit interaction on the surface of the freestanding atomically thin crystals. We find that it is not necessary to involve the effective refractive index to describe the spin-orbit interaction and the photonic SHE in the atomically thin crystals. The strong spin-orbit interaction and giant photonic SHE are predicted, which can be explained as the large polarization rotation of plane-wave components in order to satisfy the transversality of photon polarization.

  18. Analytical investigation of surface plasmon excitation on a graphene sheet using four-wave mixing.

    Science.gov (United States)

    Jamalpoor, Kamal; Zarifkar, Abbas

    2017-01-20

    In the present paper, the general conditions for exciting graphene surface plasmon polaritons (GSPPs) on a suspended graphene using nonlinear optics are investigated. The approach uses the Green's function analysis to derive GSPP fields generated under the basis of momentum conservation using four-wave mixing (FWM). Since the incident beam polarization is challenging in the nonlinear excitation of GSPPs, the significant target of this paper has been set to achieve the conditions for the third-order susceptibility tensor and the wave vectors so that the incident beams with varied polarizations are able to excite GSPPs. Nonlinear optics, in particular FWM, is utilized to compensate the mismatch between the free-space and GSPPs wave vectors. In addition, it avoids the need for applying any patterning or lithography on graphene or its substrate.

  19. Spatial distribution of spin polarization in a channel on the surface of a topological insulator.

    Science.gov (United States)

    Zhou, Xiaoying; Shao, Huaihua; Liu, Yiman; Tang, Dongsheng; Zhou, Guanghui

    2012-05-09

    We study the spatial distribution of electron spin polarization for a gate-controlled T-shaped channel on the surface of a three-dimensional topological insulator (3D TI). We demonstrate that an energy gap depending on channel geometry parameters is definitely opened due to the spatial confinement. Spin surface locking in momentum space for a uniform wide channel with Hamiltonian linearity in the wavevector is still kept, but it is broken with Hamiltonian nonlinearity in the wavevector, like that for two-dimensional surface states widely studied in the literature. However, the spin surface locking for a T-shaped channel is broken even with Hamiltonian linearity in the wavevector. Interestingly, the magnitude and direction of the in-plane spin polarization are spatially dependent in all regions due to the breaking of translational symmetry of the T-shaped channel system. These interesting findings for an electrically controlled nanostructure based on the 3D TI surface may be testable with the present experimental technique, and may provide further understanding the nature of 3D TI surface states.

  20. Energy and angular distributions of excited rhodium atoms ejected from the rhodium (100) surface

    Energy Technology Data Exchange (ETDEWEB)

    El-Maazawi, M.; Maboudian, R.; Postawa, Z.; Winograd, N. (Department of Chemistry, The Pennsylvania State University, University Park, Pennsylvania 16802 (US))

    1991-05-15

    Multiphoton resonance ionization spectroscopy has been used to determine the polar-angle and the kinetic-energy distribution of Rh atoms desorbed from the ion-bombarded Rh{l brace}100{r brace} surface in the fine-structure components of the {ital a}{sup 4}{ital F}{sub {ital J}} ground-state multiplet ({ital J}=9/2 and 7/2). The overall behavior is found to be very similar to that observed for higher-lying metastable levels. The energy distribution of the metastable level ({sup 4}{ital F}{sub 7/2} with excitation energy of {similar to}0.2 eV) is found to be broader than the ground-state ({sup 4}{ital F}{sub 9/2}) distribution. The energy distribution of the excited ejected atoms is shown to depend mainly on the electron configuration of the excited state. The measured spectra have also been used to investigate the dependence of the excitation probability on the emission velocity. It is shown that the excitation probability depends strongly on this parameter, approaching an exponential dependence on the reciprocal of the normal component of velocity at higher velocities ({gt}5{times}10{sup 5} cm/sec).

  1. Remote-excitation and remote-detection of single quantum dot using propagating surface plasmons on silver nanowire

    CERN Document Server

    Li, Qiang; Xu, Hong-Xing

    2014-01-01

    Using propagating surface plasmons (SPs) on silver nanowire (NW), we demonstrate that focused laser light at the end of silver nanowire can excite single quantum dot (QD) microns away from the excitation spot. The QD-NW interaction allows the excited QD convert part of its energy into propagating SPs which then can be detected at the remote sites. Simultaneous multi-QDs remote-excitation and detection are also realized. Furthermore, the tight confinement of propagating SPs around the NW surface enables selective excitation of QDs very close in space, which cannot be realized under conventional excitation condition. This remote excitation and detection approach may find applications in optical imaging and sensing of chemical and biological systems.

  2. Interpreting current-induced spin polarization in topological insulator surface states

    Science.gov (United States)

    Li, Pengke; Appelbaum, Ian

    2016-06-01

    Several recent experiments on three-dimensional topological insulators claim to observe a large charge current-induced nonequilibrium ensemble spin polarization of electrons in the helical surface state. We present a comprehensive criticism of such claims, using both theory and experiment: First, we clarify the interpretation of quantities extracted from these measurements by deriving standard expressions from a Boltzmann transport equation approach in the relaxation-time approximation at zero and finite temperature to emphasize our assertion that, despite high in-plane spin projection, obtainable current-induced ensemble spin polarization is minuscule. Second, we use a simple experiment to demonstrate that magnetic field-dependent open-circuit voltage hysteresis (identical to those attributed to current-induced spin polarization in topological insulator surface states) can be generated in analogous devices where current is driven through thin films of a topologically trivial metal. This result ipso facto discredits the naive interpretation of previous experiments with TIs, which were used to claim observation of helicity, i.e., spin-momentum locking in the topologically protected surface state.

  3. Coupling of surface plasmons and excited optical modes in metal/dielectric grating stacks.

    Science.gov (United States)

    Fan, Ren-Hao; Qi, Dong-Xiang; Hu, Qing; Qin, Ling; Peng, Ru-Wen; Wang, Mu

    2013-02-01

    In this work, we investigate the coupling of surface plasmons and excited optical modes in metal/dielectric grating stacks theoretically and experimentally. We have observed three kinds of modes in these structures: the cavity mode, the propagated surface plasmon (PSP) mode and the localized surface plasmon (LSP) mode, which can enhance the optical transmission. Firstly, it is shown that the cavity mode is excited in the grating stacks. And the cavity mode has redshift if we enhance the thickness of metal layers, while it has blueshift when we increase the thickness of dielectric layers. The redshift of the cavity mode also occurs when the number of repeating layers is increased. Secondly, the PSP mode is also excited, which can be described by the effective permittivity method. It is found that the PSP modes are coupled with each other, which leads to a modified dispersion relation of surface plasmon polaritons (SPP). The theoretical analysis is in good agreement with the observed transmission enhancement in the grating stacks. And the coupling of PSPs also leads to a blueshift when the number of metal layers is increased. Thirdly, the LSP mode, generated in single metal strip, can also enhance the optical transmission of the grating stacks. Yet the transmission intensity induced by LSP decreases rapidly with increasing the number of metal layers. The investigations here may have potential applications in designing plasmonic metamaterials and subwavelength optical devices.

  4. Numerical analysis of surface plasmons excited on a thin metal grating

    Institute of Scientific and Technical Information of China (English)

    OKUNO Yoichi; SUYAMA Taikei

    2006-01-01

    The authors numerically investigated the characteristics of surface plasmons excited on a thin metal grating placed in planer or conical mounting. After formulating the problem, the solution method, Yasuura's method (a modal expansion approach with least-squares boundary matching) was described. Although the grating is periodic in one direction, coupling between TE and TM waves occurs because arbitrary incidence is assumed. This requires the employment of both TE and TM vector modal functions in the analysis. Numerical computations showed: (1) the excitation of surface plasmons with total or partial absorption of incident light; (2) the resonance character of the coefficient of an evanescent order that couples the plasmon surface wave; (3) the field profile and Poynting's vector. The plasmons excited on the surfaces of a thin metal grating are classified into three types:SISP, SRSP, and LRSP, different from each other in the feature of field profile and energy flow. In addition, the eigenvalue of a plasmon mode was obtained by solving a sequence of diffraction problems with complex-valued angles of incidence and using thequasi-Newton algorithm to predict the real angle of incidence at which the absorption occurs.

  5. Excitation of surface plasmon polaritons by electron beam with graphene ribbon arrays

    Science.gov (United States)

    Liu, Yong-Qiang; Liu, Pu-Kun

    2017-03-01

    Graphene has emerged as an alternative material to support surface plasmon polaritons (SPPs) with its excellent properties such as the tight electromagnetic field localization, low dissipative loss, and versatile tunability. Thus, graphene surface plasmon polaritons (GSPs) provide an exciting platform to develop a series of novel devices and systems from the optical band to the terahertz (THz) band. In this paper, theoretical and simulated studies about the excitation of SPPs by an injected electron beam with periodic graphene ribbon arrays deposited on a dielectric medium are presented. The analytical dispersion expression of the GSP mode on the graphene ribbon arrays is obtained by using a modal expansion method along with periodic boundary conditions in the structure. With this result, the dispersion relation, propagation loss, and field pattern of the propagating GSPs for both periodic graphene microribbon arrays and the complete graphene sheet are investigated and analyzed in the THz band. It is shown that the electromagnetic field with a better concentration on the interface can be realized with graphene ribbon arrays compared with the graphene sheet for a given frequency. Besides, the excitation of GSPs by an injected electron beam with graphene ribbon arrays is modeled and implemented by the particle-in-cell simulation based on the finite difference time domain algorithm. GSPs can be excited effectively when the dispersion line of the electron beam and SPPs on the graphene ribbon arrays is matched with each other well. Besides, the dependences of output power on electron beam parameters such as the distance of the electron beam above the graphene ribbon surface and beam voltage are studied and analyzed. Finally, the tunability of graphene conductivity via biased voltage with a ground metal is considered and the tunable excitation of GSPs on the structure with biased drive voltage by the injected electron beam is also realized. The present work can find a

  6. Disentanglement of surface and bulk Rashba spin splittings in noncentrosymmetric BiTeI.

    Science.gov (United States)

    Landolt, Gabriel; Eremeev, Sergey V; Koroteev, Yury M; Slomski, Bartosz; Muff, Stefan; Neupert, Titus; Kobayashi, Masaki; Strocov, Vladimir N; Schmitt, Thorsten; Aliev, Ziya S; Babanly, Mahammad B; Amiraslanov, Imamaddin R; Chulkov, Evgueni V; Osterwalder, Jürg; Dil, J Hugo

    2012-09-14

    BiTeI has a layered and noncentrosymmetric structure where strong spin-orbit interaction leads to a giant Rashba spin splitting in the bulk bands. We present direct measurements of the bulk band structure obtained with soft x-ray angle-resolved photoemission (ARPES), revealing the three-dimensional Fermi surface. The observed spindle torus shape bears the potential for a topological transition in the bulk by hole doping. Moreover, the bulk electronic structure is clearly disentangled from the two-dimensional surface electronic structure by means of high-resolution and spin-resolved ARPES measurements in the ultraviolet regime. All findings are supported by ab initio calculations.

  7. Controlling multipolar surface plasmon excitation through the azimuthal phase structure of electron vortex beams

    Science.gov (United States)

    Ugarte, Daniel; Ducati, Caterina

    2016-05-01

    We have theoretically studied how the azimuthal phase structure of an electron vortex beam excites surface plasmons on metal particles of different geometries as observed in electron energy loss spectroscopy (EELS). We have developed a semiclassical approximation combining a ring-shaped beam and the dielectric formalism. Our results indicate that for the case of total orbital angular momentum transfer, we can manipulate surface plasmon multipole excitation and even attain an enhancement factor of several orders of magnitude. Since electron vortex beams interact with particles mostly through effects due to azimuthal symmetry, i.e., in the plane perpendicular to the electron beam, anisotropy information (longitudinal and transversal) of the sample may be derived in EELS studies by comparing nonvortex and vortex beam measurements.

  8. Tunable topological insulators with a single spin-polarized surface Dirac cone

    Science.gov (United States)

    Hsieh, David

    2010-03-01

    The topological insulator is a fundamentally new time-reversal-invariant topologically ordered phase of matter, which exhibits exotic quantum-Hall-like behavior even in the absence of an applied magnetic field. These materials are characterized by a spin-orbit coupling induced bulk energy gap and an odd number of spin-polarized Dirac cones localized on their surfaces. In this talk, I will review the first experimental realization of the topological insulator in Bi1-xSbx [1,2], and then report our recent experimental discovery and findings of a new generation of topological insulators with order-of-magnitude larger bulk band gaps and a single spin-helical surface Dirac cone [3,4]. I will also discuss a novel `effective gating' technique that can be used to optimize the insulating properties of the bulk, and to tune the Dirac carrier density on the surfaces of these new topological insulators [5]. These experiments pave the way for future transport based studies of topological insulator devices, and offer the potential for a graphene-like revolution to take place for topological insulators. [1] ``A topological Dirac insulator in a quantum spin Hall phase'', D. Hsieh et al., Nature 452, 970 (2008). [2] ``Observation of unconventional quantum spin textures in topological insulators'', D. Hsieh et al., Science 323, 919 (2009). [3] ``Observation of a large-gap topological-insulator class with a single Dirac cone on the surface'', Y. Xia et al., Nature Phys. 5, 398 (2009). [4] ``Observation of time-reversal-protected single-Dirac-cone topological-insulator states in Bi2Te3 and Sb2Te3'', D. Hsieh et al., Phys. Rev. Lett., 103, 146401 (2009). [5] ``A tunable topological insulator in the spin helical Dirac transport regime'', D. Hsieh et al., Nature 460, 1101 (2009).

  9. Electron-hole interaction and optical excitations in solids, surfaces, and polymers

    OpenAIRE

    Louie, S. G.

    2001-01-01

    The optical properties of a variety of materials have been calculated using a recently developed ab initio method based on solving the Bethe-Salpeter equation of the two-particle Green's functions. Relevant self-energy and electron-hole interaction effects are included from first-principles. Results on selected semiconductors, insulators, surfaces, and conjugated polymers are discussed. In many of these systems, excitonic effects are shown to dramatically alter the excitation energies a...

  10. Electron-hole interaction and optical excitations in solids, surfaces, and polymers

    OpenAIRE

    Louie, S. G.

    2001-01-01

    The optical properties of a variety of materials have been calculated using a recently developed ab initio method based on solving the Bethe-Salpeter equation of the two-particle Green's functions. Relevant self-energy and electron-hole interaction effects are included from first-principles. Results on selected semiconductors, insulators, surfaces, and conjugated polymers are discussed. In many of these systems, excitonic effects are shown to dramatically alter the excitation energies a...

  11. Time Dependent Coupled Cluster Approach to Resonance Raman Excitation Profiles from General Anharmonic Surfaces

    Directory of Open Access Journals (Sweden)

    M. Durga Prasad

    2002-05-01

    Full Text Available Abstract: A time dependent coupled cluster approach to the calculation of Resonance Raman excitation profiles on general anharmonic surfaces is presented. The vibrational wave functions on the ground electronic surface are obtained by the coupled cluster method (CCM. It is shown that the propagation of the vibrational ground state on the upper surface is equivalent to propagation of the vacuum state by an effective hamiltonian generated by the similarity transformation of the vibrational hamiltonian of that surface by the CCM wave operator of the lower surface up to a normalization constant. This time propagation is carried out by the time-dependent coupled cluster method in a time dependent frame. Numerical studies are presented to asses the validity of the approach.

  12. A numerical simulation of surface wave excitation in a rectangular planar-type plasma source

    Institute of Scientific and Technical Information of China (English)

    Chen Zhao-Quan; Liu Ming-Hai; Lan Chao-Hui; Chen Wei; Tang Liang; Luo Zhi-Qing; Yan Bao-Rong; Lu Jian-Hong; Hu Xi-Wei

    2009-01-01

    The principle of surface wave plasma discharge in a rectangular cavity is introduced simply based on surface plasmon polariton theory.The distribution of surface-wave electric field at the interface of the plasma-dielectric slab is investigated by using the three-dimensional finite-difference time-domain method (3D-FDTD) with different slotantenna structures.And the experimental image of discharge with a novel slot antenna array and the simulation of the electric field with this slot antenna array are both displayed.Combined with the distribution of surface wave excitation and experimental results,the numerical simulation performed by using 3D-FDTD is shown to be a useful tool in the computer-aided antenna design for large area planar-type surface-wave plasma sources.

  13. Excitation of surface electromagnetic waves in a graphene-based Bragg grating.

    Science.gov (United States)

    Sreekanth, Kandammathe Valiyaveedu; Zeng, Shuwen; Shang, Jingzhi; Yong, Ken-Tye; Yu, Ting

    2012-01-01

    Here, we report the fabrication of a graphene-based Bragg grating (one-dimensional photonic crystal) and experimentally demonstrate the excitation of surface electromagnetic waves in the periodic structure using prism coupling technique. Surface electromagnetic waves are non-radiative electromagnetic modes that appear on the surface of semi-infinite 1D photonic crystal. In order to fabricate the graphene-based Bragg grating, alternating layers of high (graphene) and low (PMMA) refractive index materials have been used. The reflectivity plot shows a deepest, narrow dip after total internal reflection angle corresponds to the surface electromagnetic mode propagating at the Bragg grating/air boundary. The proposed graphene based Bragg grating can find a variety of potential surface electromagnetic wave applications such as sensors, fluorescence emission enhancement, modulators, etc.

  14. Effects of impurities and vortices on the low-energy spin excitations in high-Tc materials

    DEFF Research Database (Denmark)

    Andersen, Brian Møller; Graser, S.; Schmid, M.

    2011-01-01

    We review a theoretical scenario for the origin of the spin-glass phase of underdoped cuprate materials. In particular it is shown how disorder in a correlated d-wave superconductor generates a magnetic phase by inducing local droplets of antiferromagnetic order which eventually merge and form a ...... disorder and/or applied magnetic fields lead to a slowing down of the dynamical spin fluctuations in agreement with neutron scattering and muon spin rotation (mSR) experiments....

  15. Excited State Potential Energy Surfaces of Polyenes and Protonated Schiff Bases.

    Science.gov (United States)

    Send, Robert; Sundholm, Dage; Johansson, Mikael P; Pawłowski, Filip

    2009-09-08

    The potential energy surface of the (1)Bu and (1)A' states of all-trans-polyenes and the corresponding protonated Schiff bases have been studied at density functional theory and coupled cluster levels. Linear polyenes and protonated Schiff bases with 4 to 12 heavy atoms have been investigated. The calculations show remarkable differences in the excited state potential energy surfaces of the polyenes and the protonated Schiff bases. The excited states of the polyenes exhibit high torsion barriers for single-bond twists and low torsion barriers for double-bond twists. The protonated Schiff bases, on the other hand, are very flexible molecules in the first excited state with low or vanishing torsion barriers for both single and double bonds. Calculations at density functional theory and coupled cluster levels yield qualitatively similar potential energy surfaces. However, significant differences are found for some single-bond torsions in longer protonated Schiff bases, which indicate a flaw of the employed time-dependent density functional theory methods. The close agreement between the approximate second and third order coupled cluster levels indicates that for these systems calculations at second order coupled cluster level are useful in the validation of results based on time-dependent density functional theory.

  16. Excitation of high-frequency surface waves with long duration in the Valley of Mexico

    Science.gov (United States)

    Iida, Masahiro

    1999-04-01

    During the 1985 Michoacan earthquake (Ms = 8.1), large-amplitude seismograms with extremely long duration were recorded in the lake bed zone of Mexico City. We interpret high-frequency seismic wave fields in the three geotechnical zones (the hill, the transition, and the lake bed zones) in the Valley of Mexico on the basis of a systematic analysis for borehole strong motion recordings. We make identification of wave types for real seismograms. First, amplitude ratios between surface and underground seismograms indicate that predominant periods of the surface seismograms are largely controlled by the wave field incident into surficial layers in the Valley of Mexico. We interpret recorded surface waves as fundamental-mode Love waves excited in the Mexican Volcanic Belt by calculating theoretical amplification for different-scale structures. Second, according to a cross-correlation analysis, the hill and transition seismograms are mostly surface waves. In the lake bed zone, while early portions are noisy body waves, late portions are mostly surface waves. Third, using two kinds of surface arrays with different station intervals, we investigate high-frequency surface-wave propagation in the lake bed zone. The wave propagation is very complicated, depending upon the time section and the frequency band. Finally, on the basis of a statistical time series model with an information criterion, we separate S- and surface-wave portions from lake bed seismograms. Surface waves are dominant and are recognized even in the early time section. Thus high-frequency surface waves with long duration in the Valley of Mexico are excited by the Mexican Volcanic Belt.

  17. Excited states of large open-shell molecules: an efficient, general, and spin-adapted approach based on a restricted open-shell ground state wave function.

    Science.gov (United States)

    Roemelt, Michael; Neese, Frank

    2013-04-11

    A spin-adapted configuration interaction with singles method that is based on a restricted open-shell reference function (ROCIS) with general total spin S is presented. All excited configuration state functions (CSFs) are generated with the aid of a spin-free second quantization formalism that only leads to CSFs within the first order interacting space. By virtue of the CSF construction, the formalism involves higher than singly excited determinants but not higher than singly excited configurations. Matrix elements between CSFs are evaluated on the basis of commutator relationships using a symbolic algebra program. The final equations were, however, hand-coded in order to maximize performance. The method can be applied to fairly large systems with more than 100 atoms in reasonable wall-clock times and also parallelizes well. Test calculations demonstrate that the approach is far superior to UHF-based configuration interaction with single excitations but necessarily falls somewhat short of quantitative accuracy due to the lack of dynamic correlation contributions. In order to implicitly account for dynamic correlation in a crude way, the program optionally allows for the use of Kohn-Sham orbitals in combination with a modest downscaling of two-electron integrals (DFT/ROCIS). All two-electron integrals of Kohn-Sham orbitals that appear in the Hamiltonian matrix are reduced by a total of three scaling parameters that are suitable for a wide range of molecules. Test calculations on open-shell organic radicals as well as transition metal complexes demonstrate the wide applicability of the method and its ability to calculate the electronic spectra of large molecular systems.

  18. A Monte Carlo study of thin spin-1 Ising films with surface exchange enhancement

    CERN Document Server

    Tucker, J W

    2000-01-01

    Using extensive Monte Carlo simulations the effect of surface exchange enhancement on ultrathin spin-1 Ising films (having simple cubic symmetry) ranging in thickness from L=3 to 8 atomic layers, has been studied. The simulations were performed on systems containing up to just over 15000 spins with periodic boundary conditions imposed in directions perpendicular to the film thickness. Within the resolution of the Monte Carlo data, it was concluded that the ratio of surface to bulk exchange interaction strengths, J sub s /J sub b) sub c sub r sub i sub t , at which the critical temperatures of the film and bulk material were equal, was independent of L, as predicted by mean field and effective field theories. However, the value of J sub s /J sub b) sub c sub r sub i sub t is spin dependent. It was found that for the spin-1 Ising films, J sub s /J sub b) sub c sub r sub i sub t =1.45, significantly below the value 1.52 obtained by Monte Carlo simulation for the spin ((1)/(2)) system reported in the literature.

  19. Vectorial mapping of noncollinear antiferromagnetic structure of semiconducting FeSe surface with spin-polarized scanning tunneling microscopy

    Energy Technology Data Exchange (ETDEWEB)

    Zhang, K. F.; Yang, Fang; Song, Y. R. [Key Laboratory of Artificial Structures and Quantum Control (Ministry of Education), Department of Physics and Astronomy, Shanghai Jiao Tong University, Shanghai 200240 (China); Zhang, Xiaole [Institute of Natural Sciences, Shanghai Jiao Tong University, Shanghai 200240 (China); The State Key Laboratory of Advanced Optical Communication Systems and Networks, Department of Physics and Astronomy, Shanghai Jiao Tong University, Shanghai 200240 (China); Chen, Xianfeng [The State Key Laboratory of Advanced Optical Communication Systems and Networks, Department of Physics and Astronomy, Shanghai Jiao Tong University, Shanghai 200240 (China); Liu, Canhua; Qian, Dong; Gao, C. L., E-mail: clgao@sjtu.edu.cn; Jia, Jin-Feng [Key Laboratory of Artificial Structures and Quantum Control (Ministry of Education), Department of Physics and Astronomy, Shanghai Jiao Tong University, Shanghai 200240 (China); Collaborative Innovation Center of Advanced Microstructures, Nanjing (China); Luo, Weidong, E-mail: wdluo@sjtu.edu.cn [Key Laboratory of Artificial Structures and Quantum Control (Ministry of Education), Department of Physics and Astronomy, Shanghai Jiao Tong University, Shanghai 200240 (China); Institute of Natural Sciences, Shanghai Jiao Tong University, Shanghai 200240 (China); Collaborative Innovation Center of Advanced Microstructures, Nanjing (China)

    2016-02-08

    Antiferromagnetic semiconductors gain increasing interest due to their possible application in spintronics. Using spin polarized scanning tunneling microscopy operating in a vector field, we mapped the noncollinear antiferromagnetic spin structure of a semiconducting hexagonal FeSe surface on the atomic scale. The surface possesses an in-plane compensated Néel structure which is further confirmed by first-principles calculations.

  20. Surface spin-glass in cobalt ferrite nanoparticles dispersed in silica matrix

    Energy Technology Data Exchange (ETDEWEB)

    Zeb, F.; Sarwer, W. [Materials Research Laboratory, Department of Physics, International Islamic University, Islamabad (Pakistan); Nadeem, K., E-mail: kashif.nadeem@iiu.edu.pk [Materials Research Laboratory, Department of Physics, International Islamic University, Islamabad (Pakistan); Kamran, M.; Mumtaz, M. [Materials Research Laboratory, Department of Physics, International Islamic University, Islamabad (Pakistan); Krenn, H. [Institute of Physics, Karl-Franzens University Graz, Universitätsplatz 5, A-8010 Graz (Austria); Letofsky-Papst, I. [Institute for Electron Microscopy, University of Technology Graz, Steyrergasse 17, A-8010 Graz (Austria)

    2016-06-01

    Surface effects in cobalt ferrite (CoFe{sub 2}O{sub 4}) nanoparticles dispersed in a silica (SiO{sub 2}) matrix were studied by using AC and DC magnetization. Nanoparticles with different concentration of SiO{sub 2} were synthesized by using sol–gel method. Average crystallite size lies in the range 25–34 nm for different SiO{sub 2} concentration. TEM image showed that particles are spherical and elongated in shape. Nanoparticles with higher concentration of SiO{sub 2} exhibit two peaks in the out-of-phase ac-susceptibility. First peak lies in the high temperature regime and corresponds to average blocking temperature of the nanoparticles. Second peak lies in the low temperature regime and is attributed to surface spin-glass freezing in these nanoparticles. Low temperature peak showed SiO{sub 2} concentration dependence and was vanished for large uncoated nanoparticles. The frequency dependence of the AC-susceptibility of low temperature peak was fitted with dynamic scaling law which ensures the presence of spin-glass behavior. With increasing applied DC field, the low temperature peak showed less shift as compared to blocking peak, broaden, and decreased in magnitude which also signifies its identity as spin-glass peak for smaller nanoparticles. M–H loops showed the presence of more surface disorder in nanoparticles dispersed in 60% SiO{sub 2} matrix. All these measurements revealed that surface effects become strengthen with increasing SiO{sub 2} matrix concentration and surface spins freeze in to spin-glass state at low temperatures. - Highlights: • Surface effects in CoFe{sub 2}O{sub 4} nanoparticles dispersed in a SiO{sub 2} matrix were studied. • Out-of-phase AC-susceptibility exhibits two peaks for SiO{sub 2} coated nanoparticles. • First peak corresponds to average blocking temperature. • Second peak is attributed to surface spin-glass freezing • The spin-glass behavior depends upon the SiO{sub 2} matrix concentration.

  1. Cherenkov terahertz surface plasmon excitation by an electron beam over an ultrathin metal film

    Science.gov (United States)

    Kumar, Pawan; Kumar, Rajeev; Rajouria, Satish Kumar

    2016-12-01

    The mechanism of Cherenkov excitation of terahertz (THz) surface plasma wave (SPW), by a relativistic electron beam propagating over an ultrathin metal film deposited on glass, is investigated. The SPW field falls off exponentially in vacuum as well as glass, while the surface plasmon resonant frequency is lowered by the reduction of film thickness. The SPW field causes density bunching of the beam leading to current modulation and generation of THz radiation via the Cherenkov interaction. The frequency of the THz decreases with the energy of the beam, whereas the growth rate increases.

  2. Efficient out-coupling and beaming of Tamm optical states via surface plasmon polariton excitation

    Energy Technology Data Exchange (ETDEWEB)

    Lopez-Garcia, M.; Ho, Y.-L. D.; Taverne, M. P. C.; Chen, L.-F.; Rarity, J. G.; Oulton, R. [Department of Electrical and Electronic Engineering, University of Bristol, Faculty of Engineering, Queen' s Building, University Walk, Bristol BS8 1TR (United Kingdom); Murshidy, M. M. [Department of Physics and Mathematics, University of Hull, Cottingham Road, HU6 7RX Hull (United Kingdom); Department of Physics, Faculty of Science, Helwan University, Helwan (Egypt); Yousef Jameel Science and Technology Research Center, The American University in Cairo (Egypt); Edwards, A. P.; Adawi, A. M. [Department of Physics and Mathematics, University of Hull, Cottingham Road, HU6 7RX Hull (United Kingdom); Serry, M. Y. [Yousef Jameel Science and Technology Research Center, The American University in Cairo (Egypt)

    2014-06-09

    We present evidence of optical Tamm states to surface plasmon polariton (SPP) coupling. We experimentally demonstrate that for a Bragg stack with a thin metal layer on the surface, hybrid Tamm-SPP modes may be excited when a grating on the air-metal interface is introduced. Out-coupling via the grating to free space propagation is shown to enhance the transmission as well as the directionality and polarization selection for the transmitted beam. We suggest that this system will be useful on those devices, where a metallic electrical contact as well as beaming and polarization control is needed.

  3. Intrinsic life-time and external manipulation of Néel states in antiferromagnetic adatom spins on semiconductor surfaces

    Science.gov (United States)

    Li, Jun; Liu, Bang-Gui

    2015-06-01

    It has been proposed that antiferromagnetic Fe adatom spins on semiconductor Cu-N surfaces can be used to store information (Loth et al 2012 Science 335 196). Here, we investigate spin dynamics of such antiferromagnetic systems through Monte Carlo simulations. We find out the temperature and size laws of switching rates of Néel states and show that the Néel states can become stable enough for the information storage when the number of spins reaches one or two dozens of the Fe spins. We also explore promising methods for manipulating the Néel states. These could help realize information storage with such antiferromagnetic spin systems.

  4. Large spin splitting of metallic surface-state bands at adsorbate-modified gold/silicon surfaces.

    Science.gov (United States)

    Bondarenko, L V; Gruznev, D V; Yakovlev, A A; Tupchaya, A Y; Usachov, D; Vilkov, O; Fedorov, A; Vyalikh, D V; Eremeev, S V; Chulkov, E V; Zotov, A V; Saranin, A A

    2013-01-01

    Finding appropriate systems with a large spin splitting of metallic surface-state band which can be fabricated on silicon using routine technique is an essential step in combining Rashba-effect based spintronics with silicon technology. We have found that originally poor structural and electronic properties of the Au/Si(111) √3 x √3 surface can be substantially improved by adsorbing small amounts of suitable species (e.g., Tl, In, Na, Cs). The resultant surfaces exhibit a highly-ordered atomic structure and spin-split metallic surface-state band with a momentum splitting of up to 0.052 Å(-1) and an energy splitting of up to 190 meV at the Fermi level. The family of adsorbate-modified Au/Si(111) √3 x √3 surfaces, on the one hand, is thought to be a fascinating playground for exploring spin-splitting effects in the metal monolayers on a semiconductor and, on the other hand, expands greatly the list of material systems prospective for spintronics applications.

  5. Regulating spin and Fermi surface topology of a quantum metal film by the surface (interface) monatomic layer

    Science.gov (United States)

    Matsuda, Iwao

    2012-02-01

    Spin and current controls in solids have been one of the central issues in researches of electron and spin transport. Nowadays, electronics/spintronics deals with nanometer- or atomic-scale structures and miniaturization of these systems implies emergence of various quantum phenomena, intimately linked to the formation of electronic states different from those of the corresponding bulk materials. For example, valence electrons of films with the thickness comparable to the electron wavelength form discrete quantum-well states (QWSs) under opportune conditions of confinement (quantum size effect). Furthermore, the size reduction also increases the surface/volume ratio and a film possibly changes its electronic (spin) properties by the surface effect. Concerning metal films, the quantum size effect requires the thickness in a range of nanometers and the length corresponds to several tens of atoms, indicating the very large ratio of a surface (interface) monatomic layer to film atomic layers. Thus, we have been interested in combining the quantum size effects and the surface effect on the metal films to induce new physical phenomena. In the present talk, two research cases are shown. 1) Instead of isotropic two-dimensional in-plane states expected for an isolated metal film, quasi-one-dimensional quantized states were measured by photoemission spectroscopy in an epitaxial Ag(111) ultra thin film, prepared on an array of atomic chains [1]. 2) High-resolution spin-resolved photoemission and magneto-transport experiments of ultrathin Ag(111) films, covered with a /3x/3-Bi/Ag surface ordered alloy, were performed. The surface state (SS) bands, spin-split by the Rashba interaction, selectively couple to the originally spin-degenerate QWS bands in the metal film, making the spin-dependent hybridization [2,3]. Magnetoconductance of the films, measured in situ by the micro-four-point probe method as a function of the applied magnetic field [4], has shown that the formation of

  6. Analysis of KLL Auger spectra excited by X-rays from Ni and Cu metal surfaces

    Science.gov (United States)

    Egri, S.; Kövér, L.; Cserny, I.; Novák, M.; Drube, W.

    2016-02-01

    Ni and Cu KLL Auger spectra excited by X-rays from polycrystalline metal foils were measured with good energy resolution and intensity earlier. Auger spectra of 3d transition metals contain satellite peaks due to the atomic excitation processes. Because of the complexity of the measured spectral shape a complete explanation of the spectra was not given in the previous works. A new analysis of the measured spectra is presented here, with improved description of effects of inelastic electron scattering of the electrons in the solid sample and using complex peak shapes to model the satellite structure that follows each diagram line. The energy loss part of measured spectra due to the bulk plasmon excitations, surface plasmon excitations and intrinsic loss processes was removed using the Partial Intensity Analysis method based on energy loss distributions obtained from experimental reflection electron energy loss spectra of the same Cu and Ni metal foils. Relative Auger-transition energies derived from measured spectra of copper are in good agreement with previous experimental works and the results of cluster molecular orbital multielectron (DV-ME) calculations. The intensity ratio I(3P2/3P0) shows better agreement with the result of relativistic calculations than in previous works. In the case of nickel the relative Auger-transition energies are in good agreement with the previous results. According to the new evaluation four satellite peaks were identified on the low energy side of each diagram line in the Auger spectra of Ni.

  7. Giant transmission Goos-Hänchen shift in surface plasmon polaritons excitation and its physical origin

    Science.gov (United States)

    Yang, Yang; Liu, Ju; Li, Zhi-Yuan

    2015-07-01

    Excitation of surface plasmon polaritons (SPPs) propagating at the interface between a dielectric medium and a silver thin film by a focused Gaussian beam in a classical Kretschmann prism setup is studied theoretically. We find that the center of the transmitted Gaussian evanescent wave has a giant lateral shift relative to the incident Gaussian beam center for a wide range of incident angle and Gaussian beam wavelength to excite SPPs, which can be more than two orders of magnitude larger than the silver film thickness. The phenomenon is closely related with the conventional Goos-Hänchen effect for total internal reflection of light beam, and it is called the transmission Goos-Hänchen shift. We find that this lateral shift depends heavily on the excitation wavelength, incident angle, and the silver layer thickness. Finite-difference time-domain simulations show that this transmission Goos-Hänchen shift is induced by a unique dynamical process of excitation, transport, and leakage of SPPs. Project supported by the National Basic Research Program of China (Grant No. 2013CB632704) and the National Natural Science Foundation of China (Grant No. 11374357).

  8. Integration of spin-state-selective excitation into 2D NMR correlation experiments with heteronuclear ZQ/2Q {pi} rotations for{sup 1} J{sub XH}

    Energy Technology Data Exchange (ETDEWEB)

    Meissner, Axel; Duus, Jens O.; Sorensen, Ole Winneche [Department of Chemistry, Carlsberg Laboratory (Denmark)

    1997-07-15

    Spin-State-Selective Excitation (S{sup 3}E), which for example selectively excites amide proton resonances corresponding to exclusively either the {alpha} or the {beta} spin state of the covalently bound {sup 15}N atom is employed for E.COSY-type extraction of heteronuclear J coupling constants. Instead of having one spectrum with two peaks (corresponding to the {alpha} or {beta} spin state of{sup 15}N), S{sup 3}E generates two spectra, each with only one peak for each {sup 15}N nucleus. These two spectra are generated from the same data set, so that there is no reduction in sensitivity compared to conventional {sup 1}J{sub NH}-resolved methods.Another interesting feature in comparison with conventional methods is that{sup 1}J{sub NH} can be suppressed during the evolution period, meaning that no heteronuclear multiplet structure is visible in the{omega}{sub 1} frequency dimension. The S{sup 3}E pulse sequence element is combined with NOESY for measurement of{sup 3}J{sub N-H{beta}} and J{sub N-H{alpha}}coupling constants in either a hetero- or a homonuclear correlated version.Experimental confirmation is obtained using the protein RAP 17-;97(N-terminal domain of {alpha}{sub 2}-macroglobulin Receptor Associated Protein)

  9. Surface-embeddability approach to the dynamics of the inhomogeneous Heisenberg spin chain

    Science.gov (United States)

    Balakrishnan, Radha; Guha, Partha

    1996-08-01

    The surface-embeddability approach of Lund and Regge is applied to the classical, inhomogeneous Heisenberg spin chain to study the class of inhomogeneity functions f for which the spin evolution equation and its gauge-equivalent generalized nonlinear Schrödinger equation (GNLSE) are exactly solvable. Writing the spin vector S(x,t) as ∂xr and identifying r(x,t) with a position vector generating a surface, we show that the kinematic equation satisfied by r implies certain constraints on the admissible geometries of this surface. These constraints, together with the Gauss-Mainardi-Codazzi equations, enable us to express the coefficient of the second fundamental form as well as f in terms of the metric coefficients G and its derivatives, for arbitrary time-independent G. Explicit solutions for the GNLSE can also be found in terms of the same quantities. Of the admissible surfaces generated by r, a special class that emerges naturally is that of surfaces of revolution: Explicit solutions for r and S are found and discussed for this class of surfaces.

  10. Two New Type Surface Polaritons Excited into Nanoholes in Metal Films

    Directory of Open Access Journals (Sweden)

    Minasyan V. N.

    2010-04-01

    Full Text Available We argue that the smooth metal-air interface should be regarded as a distinct dielectric medium, the skin of the metal. Here we present quantized Maxwell’s equations for electromagnetic field in an isotropic homogeneous medium, allowing us to solve the absorption anomaly property of these metal films. The results imply the existence of light quasi-particles with spin one and effective mass m = 2.5 E-5 me which in turn provide the presence of two type surface polaritons into nanoholes in metal films.

  11. The spin chemistry and magnetic resonance of H2@C60. From the Pauli principle to trapping a long lived nuclear excited spin state inside a buckyball.

    Science.gov (United States)

    Turro, Nicholas J; Chen, Judy Y-C; Sartori, Elena; Ruzzi, Marco; Marti, Angel; Lawler, Ronald; Jockusch, Steffen; López-Gejo, Juan; Komatsu, Koichi; Murata, Yasujiro

    2010-02-16

    One of the early triumphs of quantum mechanics was Heisenberg's prediction, based on the Pauli principle and wave function symmetry arguments, that the simplest molecule, H(2), should exist as two distinct species-allotropes of elemental hydrogen. One allotrope, termed para-H(2) (pH(2)), was predicted to be a lower energy species that could be visualized as rotating like a sphere and possessing antiparallel ( upward arrow downward arrow) nuclear spins; the other allotrope, termed ortho-H(2) (oH(2)), was predicted to be a higher energy state that could be visualized as rotating like a cartwheel and possessing parallel ( upward arrow upward arrow) nuclear spins. This remarkable prediction was confirmed by the early 1930s, and pH(2) and oH(2) were not only separated and characterized but were also found to be stable almost indefinitely in the absence of paramagnetic "spin catalysts", such as molecular oxygen, or traces of paramagnetic impurities, such as metal ions. The two allotropes of elemental hydrogen, pH(2) and oH(2), may be quantitatively incarcerated in C(60) to form endofullerene guest@host complexes, symbolized as pH(2)@C(60) and oH(2)@C(60), respectively. How does the subtle difference in nuclear spin manifest itself when hydrogen allotropes are incarcerated in a buckyball? Can the incarcerated "guests" communicate with the outside world and vice versa? Can a paramagnetic spin catalyst in the outside world cause the interconversion of the allotropes and thereby effect a chemical transformation inside a buckyball? How close are the measurable properties of H(2)@C(60) to those computed for the "quantum particle in a spherical box"? Are there any potential practical applications of this fascinating marriage of the simplest molecule, H(2), with one of the most beautiful of all molecules, C(60)? How can one address such questions theoretically and experimentally? A goal of our studies is to produce an understanding of how the H(2) guest molecules incarcerated in

  12. Coupling between magnetic field and curvature in Heisenberg spins on surfaces with rotational symmetry

    Energy Technology Data Exchange (ETDEWEB)

    Carvalho-Santos, Vagson L., E-mail: vagson.santos@ufv.br [Instituto Federal de Educação, Ciência e Tecnologia Baiano, Campus Senhor do Bonfim, 48970-000 Senhor do Bonfim, Bahia (Brazil); Dandoloff, Rossen [Laboratoire de Physique Théorique et Modélisation, Université de Cergy-Pontoise, 95302 Cergy-Pontoise (France)

    2012-10-15

    We study the nonlinear σ-model in an external magnetic field applied on curved surfaces with rotational symmetry. The Euler–Lagrange equations derived from the Hamiltonian yield the double sine-Gordon equation (DSG) provided the magnetic field is tuned with the curvature of the surface. A 2π skyrmion appears like a solution for this model and surface deformations are predicted at the sector where the spins point in the opposite direction to the magnetic field. We also study some specific examples by applying the model on three rotationally symmetric surfaces: the cylinder, the catenoid and the hyperboloid.

  13. Microscopic study of edge excitations of spin-polarized and spin-unpolarized ν=2/3 fractional quantum Hall effect

    Science.gov (United States)

    Wu, Ying-Hai; Sreejith, G. J.; Jain, Jainendra K.

    2012-09-01

    The edge of spin-unpolarized or spin-polarized ν=2/3 fractional quantum Hall states is predicted by the effective theory to support a backward-moving neutral mode in addition to a forward-moving charge mode. We study this issue from a microscopic perspective where these states are identified with an effective filling factor of 2 of composite fermions, but with an effective magnetic field that is antiparallel to the external field. A simple counting from the composite fermion description suggests that there might be two backward-moving edge modes, but explicit calculations show that one of these is projected out of the low-energy sector, while the remaining mode provides a good microscopic account of the actual counterpropagating edge mode. The forward-moving modes are identified as “Schur modes,” obtained by multiplying the ground-state wave function by the symmetric Schur polynomials. The edge of the 2/3 spin unpolarized state provides a particularly striking realization of “spin-charge separation” in one-dimensional Tomonaga-Luttinger liquids, with the spin and charge modes moving in opposite directions.

  14. Quantum model of a solid-state spin qubit: Ni cluster on a silicon surface by the generalized spin Hamiltonian and X-ray absorption spectroscopy investigations

    Energy Technology Data Exchange (ETDEWEB)

    Farberovich, Oleg V. [School of Physics and Astronomy, Beverly and Raymond Sackler Faculty of Exact Sciences, Tel Aviv University, Tel Aviv 69978 (Israel); Research Center for Nanoscale Structure of Matter, Southern Federal University, Zorge 5, 344090 Rostov-on-Don (Russian Federation); Voronezh State University, Voronezh 394000 (Russian Federation); Mazalova, Victoria L., E-mail: mazalova@sfedu.ru [Research Center for Nanoscale Structure of Matter, Southern Federal University, Zorge 5, 344090 Rostov-on-Don (Russian Federation); Soldatov, Alexander V. [Research Center for Nanoscale Structure of Matter, Southern Federal University, Zorge 5, 344090 Rostov-on-Don (Russian Federation)

    2015-11-15

    We present here the quantum model of a Ni solid-state electron spin qubit on a silicon surface with the use of a density-functional scheme for the calculation of the exchange integrals in the non-collinear spin configurations in the generalized spin Hamiltonian (GSH) with the anisotropic exchange coupling parameters linking the nickel ions with a silicon substrate. In this model the interaction of a spin qubit with substrate is considered in GSH at the calculation of exchange integrals J{sub ij} of the nanosystem Ni{sub 7}–Si in the one-electron approach taking into account chemical bonds of all Si-atoms of a substrate (environment) with atoms of the Ni{sub 7}-cluster. The energy pattern was found from the effective GSH Hamiltonian acting in the restricted spin space of the Ni ions by the application of the irreducible tensor operators (ITO) technique. In this paper we offer the model of the quantum solid-state N-spin qubit based on the studying of the spin structure and the spin-dynamics simulations of the 3d-metal Ni clusters on the silicon surface. The solution of the problem of the entanglement between spin states in the N-spin systems is becoming more interesting when considering clusters or molecules with a spectral gap in their density of states. For quantifying the distribution of the entanglement between the individual spin eigenvalues (modes) in the spin structure of the N-spin system we use the density of entanglement (DOE). In this study we have developed and used the advanced high-precision numerical techniques to accurately assess the details of the decoherence process governing the dynamics of the N-spin qubits interacting with a silicon surface. We have studied the Rabi oscillations to evaluate the N-spin qubits system as a function of the time and the magnetic field. We have observed the stabilized Rabi oscillations and have stabilized the quantum dynamical qubit state and Rabi driving after a fixed time (0.327 μs). The comparison of the energy

  15. Optically tunable spin transport on the surface of a topological insulator

    Science.gov (United States)

    Yudin, D.; Kibis, O. V.; Shelykh, I. A.

    2016-10-01

    The emerging field of spinoptronics has a potential to supersede the functionality of modern electronics, while a proper description of strong light-matter coupling pose the most intriguing questions from both fundamental scientific and technological perspectives. In this paper we address a highly relevant issue for such a development. We theoretically explore spin dynamics on the surface of a 3D topological insulator (TI) irradiated with an off-resonant high-frequency electromagnetic wave. The strong coupling between electrons and the electromagnetic wave drastically modifies the spin properties of TI. The effects of irradiation are shown to result in anisotropy of electron energy spectrum near the Dirac point and suppression of spin current and are investigated in detail in this work.

  16. Properties of Surface Plasmon Polaritons on lossy materials: Lifetimes, periods and excitation conditions

    CERN Document Server

    Derrien, Thibault J -Y; Bonse, Jörn

    2016-01-01

    The possibility to excite Surface Plasmon Polaritons (SPPs) at the interface between two media depends on the optical properties of both media and geometrical aspects. Specific conditions allowing the coupling of light with a plasmon-active interface must be satisfied. Plasmonic effects are well described in noble metals where the imaginary part of the dielectric permittivity is often neglected ("perfect medium approximation"). However, some systems exist for which such approximation cannot be applied, hence requiring a refinement of the common SPP theory. In this context, several properties of SPPs such as excitation conditions, period of the electromagnetic field modulation and SPP lifetime then may strongly deviate from that of the perfect medium approximation. In this paper, calculations taking into account the imaginary part of the dielectric permittivities are presented. The model identifies analytical terms which should not be neglected in the mathematical description of SPPs on lossy materials. These ...

  17. Coupling-induced excitation of a forbidden surface plasmon mode of a gold nanorod

    Institute of Scientific and Technical Information of China (English)

    YAO HaoMin; LI Zhi; GONG QiHuang

    2009-01-01

    Using the finite-difference time-domain (FDTD) method, we simulate the coupling between a gold nanorod and gold nanoparticles with different plasmonic resonant frequencies/volumes as well as that between the nanorod and a dielectric nanosphere. The influences of coupling with different nanoparti-cles on the excitation of a forbidden longitudinal surface plasmon mode of the nanorod under normal incidence are investigated. It is found that the cause of this excitation is the broken symmetry of the local electric field experienced by the nanorod resulting from the charge pileup on the other nanopar-ticle. This result is valuable for understanding the near-field optical characterization of plasmonic metal nanoparticles.

  18. Coupling-induced excitation of a forbidden surface plasmon mode of a gold nanorod

    Institute of Scientific and Technical Information of China (English)

    2009-01-01

    Using the finite-difference time-domain(FDTD) method,we simulate the coupling between a gold nanorod and gold nanoparticles with different plasmonic resonant frequencies/volumes as well as that between the nanorod and a dielectric nanosphere.The influences of coupling with different nanoparticles on the excitation of a forbidden longitudinal surface plasmon mode of the nanorod under normal incidence are investigated.It is found that the cause of this excitation is the broken symmetry of the local electric field experienced by the nanorod resulting from the charge pileup on the other nanoparticle.This result is valuable for understanding the near-field optical characterization of plasmonic metal nanoparticles.

  19. Nanowires-assisted excitation and propagation of mid-infrared surface plasmon polaritons in graphene

    Science.gov (United States)

    Lu, Hua; Zhao, Jianlin; Gu, Min

    2016-10-01

    We investigate the excitation and propagation of surface plasmon polaritons in a novel graphene hybrid photonic nanostructure, which consists of a graphene sheet and a dielectric layer with partly etched nanowires coated on the silicon substrate. The simulation and analytical results show that the mid-infrared plasmonic wave can be generated in the graphene sheet by normally incident light due to the satisfaction of the wavevector matching condition. Especially, we find that the plasmonic wavelength and spectral width are determined by the width, pitch, and refractive index of the dielectric nanowires, as well as the layer number and the Fermi level of graphene sheet. The analytical calculations agree well with the finite-difference time-domain simulations. These results would provide an new avenue toward the excitation of graphene plasmonics for the manipulation of mid-infrared light at nanoscale.

  20. A matrix model for strings beyond the c=1 barrier: the spin-s Heisenberg model on random surfaces

    CERN Document Server

    Ambjorn, J; Sedrakyan, A

    2014-01-01

    We consider a spin-s Heisenberg model coupled to two-dimensional quantum gravity. We quantize the model using the Feynman path integral, summing over all possible two-dimensional geometries and spin configurations. We regularize this path integral by starting with the R-matrices defining the spin-s Heisenberg model on a regular 2d Manhattan lattice. 2d quantum gravity is included by defining the R-matrices on random Manhattan lattices and summing over these, in the same way as one sums over 2d geometries using random triangulations in non-critical string theory. We formulate a random matrix model where the partition function reproduces the annealed average of the spin-s Heisenberg model over all random Manhattan lattices. A technique is presented which reduces the random matrix integration in partition function to an integration over their eigenvalues.

  1. Surface optomechanics: Calculating optically excited acoustical whispering gallery modes in microspheres

    CERN Document Server

    Zehnpfennig, John; Tomes, Matthew; Carmon, Tal

    2011-01-01

    Stimulated Brillouin scattering recently allowed experimental excitation of surface acoustic resonances in micro-devices, enabling vibration at rates in the range of 50 MHz to 12 GHz. The experimental availability of such mechanical whispering gallery modes in photonic-MEMS raises questions on their structure and spectral distribution. Here we calculate the form and frequency of such vibrational surface whispering gallery modes, revealing diverse types of surface vibrations including longitudinal, transverse, and Rayleigh-type deformations. We parametrically investigate these various modes by changing their orders in the azimuthal, radial, and polar directions to reveal different vibrational structures including mechanical resonances that are localized near the interface with the environment where they can sense changes in the surroundings.

  2. Excitation of surface waves on the interfaces of general bi-isotropic media

    CERN Document Server

    Kim, Seulong

    2016-01-01

    We study theoretically the characteristics of surface waves excited at the interface between a metal and a general bi-isotropic medium, which includes isotropic chiral media and Tellegen media as special cases. We derive an analytical dispersion relation for surface waves, using which we calculate the effective index and the propagation length numerically. We also calculate the absorptance, the cross-polarized reflectance and the spatial distribution of the electromagnetic fields for plane waves incident on a bilayer system consisting of a metal layer and a bi-isotropic layer in the Kretschmann configuration, using the invariant imbedding method. The results obtained using the invariant imbedding method agree with those obtained from the dispersion relation perfectly. In the case of chiral media, the effective index is an increasing function of the chirality index, whereas in Tellegen media, it is a decreasing function of the Tellegen parameter. The propagation length for surface waves in both cases increase ...

  3. Inelastic light scattering by electrons in GaAs quantum wires: Spin-density, charge-density and single-particle excitations

    Science.gov (United States)

    Schmeller, A.; Goñi, A. R.; Pinczuk, A.; Weiner, J. S.; Calleja, J. M.; Dennis, B. S.; Pfeiffer, L. N.; West, K. W.

    1994-06-01

    In inelastic light scattering experiments we observe for the first time clearly resolved one dimensional (1D) intersubband spin-density excitations. Together with new structure at energies close to the 2D intersubband transitions, these observations display the formation of 1D subbands. The depolarization shift ( Wdep) and the excitonic shift ( Wxc) can be deduced approximately from our experiments. These shifts are of special interest because they are related to the direct and exchange-correlation terms of the electron-electron interaction. We find ratios of the shifts ( Wxc/ Wdep) of up to 55%.

  4. Excitation of surface plasma waves over corrugated slow-wave structure

    Indian Academy of Sciences (India)

    Ashim P Jain; Jetendra Parashar

    2005-08-01

    A microwave propagating along vacuum–dielectric–plasma interface excites surface plasma wave (SPW). A periodic slow-wave structure placed over dielectric slows down the SPW. The phase velocity of slow SPW is sensitive to height, periodicity, number of periods, thickness and the separation between dielectric and slow-wave structure. These slow SPW can couple the microwave energy to the plasma and can sustain the discharge. The efficiency of the power coupling is few per cent and is sensitive to separation between dielectric and slow-wave structure.

  5. Direct observation of surface mode excitation and slow light coupling in photonic crystal waveguides

    DEFF Research Database (Denmark)

    Volkov, V.S.; Bozhevolnyi, Sergey I.; Frandsen, Lars Hagedorn;

    2007-01-01

    are obtained for light at telecom wavelengths propagating in the PhCW, demonstrating directly, for the first time to our knowledge, drastic widening of the PhCW guided mode in the slow-light regime and excitation of surface waves at the PhCW interface along with their feeding into the guided mode......A scanning near-field optical microscope (SNOM) is used to systematically study the properties of guided modes in linear and slow-light regimes of silicon-on-insulator (SOI)-based photonic crystal waveguides (PhCWs) with different terminations of the photonic lattice. High quality SNOM images...

  6. Control and characterization of spatio-temporal disorder in parametrically excited surface waves

    Indian Academy of Sciences (India)

    T Epsteing; J Fineberg

    2005-06-01

    The nonlinear interactions of parametrically excited surface waves have been shown to yield a rich family of nonlinear states. When the system is driven by two commensurate frequencies, a variety of interesting superlattice type states are generated via a number of different 3-wave resonant interactions. These states occur either as symmetry-breaking bifurcations of hexagonal patterns composed of a single unstable mode or via nonlinear interactions between the two different unstable modes generated by the two forcing frequencies. Near the system’s bicritical point, a well-defined region of phase space exists in which a highly disordered state, both in space and time, is observed. We first show that this state results from the competition between two distinct nonlinear superlattice states, each with different characteristic temporal and spatial symmetries. After characterizing the type of spatio-temporal disorder that is embodied in this disordered state, we will demonstrate that it can be controlled. Control to either of its neighboring nonlinear states is achieved by the application of a small-amplitude excitation at a third frequency, where the spatial symmetry of the selected pattern is determined by the temporal symmetry of the third frequency used. This technique can also excite rapid switching between different nonlinear states.

  7. Laser Raman Spectroscopy with Different Excitation Sources and Extension to Surface Enhanced Raman Spectroscopy

    Directory of Open Access Journals (Sweden)

    Md. Wahadoszamen

    2015-01-01

    Full Text Available A dispersive Raman spectrometer was used with three different excitation sources (Argon-ion, He-Ne, and Diode lasers operating at 514.5 nm, 633 nm, and 782 nm, resp.. The system was employed to a variety of Raman active compounds. Many of the compounds exhibit very strong fluorescence while being excited with a laser emitting at UV-VIS region, hereby imposing severe limitation to the detection efficiency of the particular Raman system. The Raman system with variable excitation laser sources provided us with a desired flexibility toward the suppression of unwanted fluorescence signal. With this Raman system, we could detect and specify the different vibrational modes of various hazardous organic compounds and some typical dyes (both fluorescent and nonfluorescent. We then compared those results with the ones reported in literature and found the deviation within the range of ±2 cm−1, which indicates reasonable accuracy and usability of the Raman system. Then, the surface enhancement technique of Raman spectrum was employed to the present system. To this end, we used chemically prepared colloidal suspension of silver nanoparticles as substrate and Rhodamine 6G as probe. We could observe significant enhancement of Raman signal from Rhodamine 6G using the colloidal solution of silver nanoparticles the average magnitude of which is estimated to be 103.

  8. Excited state potential energy surfaces of bistridentate RuII complexes - A TD-DFT study

    Science.gov (United States)

    Österman, Tomas; Persson, Petter

    2012-10-01

    Time-dependent density functional theory (TD-DFT) calculations have been used to investigate low-energy singlet and triplet excited state potential energy surfaces (PES) of two prototype RuII-bistridentate complexes: [RuII(tpy)2]2+ (tpy is 2,2':6',2''-terpyridine) and [RuII(dqp)2]2+ (dqp is 2,6-di(quinolin-8-yl)pyridine). Solvent effects were considered using a self-consistent reaction field scheme. The calculations provide information about the excited state manifold along pathways for activated decay of metal-to-ligand charge-transfer (MLCT) excited states via metal-centered (MC) states for the two complexes. Significant differences in the energy profiles of the investigated PESs are explained through characterization of the electronic properties of the involved states calculated by the TD-DFT calculations. Finally, implications of the computational results for the design of octahedral metal complexes utilizing ligand field splitting (LFS) strategies for efficient light-harvesting in photochemical applications such as artificial photosynthesis are discussed.

  9. Surface plasmons excited by the photoluminescence of organic nanofibers in hybrid plasmonic systems

    Science.gov (United States)

    Sobolewska, ElŻbieta K.; Leißner, Till; Jozefowski, Leszek; Brewer, Jonathan; Rubahn, Horst-Günter; Adam, Jost; Fiutowski, Jacek

    2016-04-01

    Recent research on hybrid plasmonic systems has shown the existence of a loss channel for energy transfer between organic materials and plasmonic/metallic structured substrates. This work focuses on the exciton-plasmon coupling between para-Hexaphenylene (p-6P) organic nanofibers (ONFs) and surface plasmon polaritons (SPPs) in organic/dielectric/metal systems. We have transferred the organic p-6P nanofibers onto a thin silver film covered with a dielectric (silicon dioxide) spacer layer with varying thicknesses. Coupling is investigated by two-photon fluorescence-lifetime imaging microscopy (FLIM) and leakage radiation spectroscopy (LRS). Two-photon excitation allows us to excite the ONFs with near-infrared light and simultaneously avoids direct SPP excitation on the metal layer. We observe a strong dependence of fluorescence lifetime on the type of underlying substrate and on the morphology of the fibers. The experimental findings are complemented via finite-difference time-domain (FDTD) modeling. The presented results lead to a better understanding and control of hybrid-mode systems, which are crucial elements in future low-loss energy transfer devices.

  10. Spin-helical Dirac states in graphene induced by polar-substrate surfaces with giant spin-orbit interaction: a new platform for spintronics.

    Science.gov (United States)

    Eremeev, S V; Nechaev, I A; Echenique, P M; Chulkov, E V

    2014-11-04

    Spintronics, or spin electronics, is aimed at efficient control and manipulation of spin degrees of freedom in electron systems. To comply with demands of nowaday spintronics, the studies of electron systems hosting giant spin-orbit-split electron states have become one of the most important problems providing us with a basis for desirable spintronics devices. In construction of such devices, it is also tempting to involve graphene, which has attracted great attention because of its unique and remarkable electronic properties and was recognized as a viable replacement for silicon in electronics. In this case, a challenging goal is to lift spin degeneracy of graphene Dirac states. Here, we propose a novel pathway to achieve this goal by means of coupling of graphene and polar-substrate surface states with giant Rashba-type spin-splitting. We theoretically demonstrate it by constructing the graphene@BiTeCl system, which appears to possess spin-helical graphene Dirac states caused by the strong interaction of Dirac and Rashba electrons. We anticipate that our findings will stimulate rapid growth in theoretical and experimental investigations of graphene Dirac states with real spin-momentum locking, which can revolutionize the graphene spintronics and become a reliable base for prospective spintronics applications.

  11. Static polarizabilities for excited states within the spin-conserving and spin-flipping equation-of-motion coupled-cluster singles and doubles formalism: Theory, implementation, and benchmarks.

    Science.gov (United States)

    Nanda, Kaushik D; Krylov, Anna I

    2016-11-28

    We present the theory and implementation for calculating static polarizabilities within the equation-of-motion coupled-cluster singles and doubles (EOM-CCSD) framework for electronically excited states and its spin-flip variant. We evaluate the second derivatives of the EOM-CCSD Lagrangian with respect to electric-field perturbations. The relaxation of reference molecular orbitals is not included. In our approach, the wave function amplitudes satisfy the 2n + 1 rule and the amplitude-response Lagrange multipliers satisfy the 2n + 2 rule. The new implementation is validated against finite-field and CCSD response-theory calculations of the excited-state polarizabilities of pyrimidine and s-tetrazine. We use the new method to compute static polarizabilities of different types of electronic states (valence, charge-transfer, singlets, and triplets) in open- and closed-shell systems (uracil, p-nitroaniline, methylene, and p-benzyne). We also present an alternative approach for calculating excited-state static polarizabilities as expectation values by using the EOM-CCSD wave functions and energies in the polarizability expression for an exact state. We find that this computationally less demanding approach may show differences up to ∼30% relative to the excited-state polarizabilities computed using the analytic-derivative formalism.

  12. Static polarizabilities for excited states within the spin-conserving and spin-flipping equation-of-motion coupled-cluster singles and doubles formalism: Theory, implementation, and benchmarks

    Science.gov (United States)

    Nanda, Kaushik D.; Krylov, Anna I.

    2016-11-01

    We present the theory and implementation for calculating static polarizabilities within the equation-of-motion coupled-cluster singles and doubles (EOM-CCSD) framework for electronically excited states and its spin-flip variant. We evaluate the second derivatives of the EOM-CCSD Lagrangian with respect to electric-field perturbations. The relaxation of reference molecular orbitals is not included. In our approach, the wave function amplitudes satisfy the 2n + 1 rule and the amplitude-response Lagrange multipliers satisfy the 2n + 2 rule. The new implementation is validated against finite-field and CCSD response-theory calculations of the excited-state polarizabilities of pyrimidine and s-tetrazine. We use the new method to compute static polarizabilities of different types of electronic states (valence, charge-transfer, singlets, and triplets) in open- and closed-shell systems (uracil, p-nitroaniline, methylene, and p-benzyne). We also present an alternative approach for calculating excited-state static polarizabilities as expectation values by using the EOM-CCSD wave functions and energies in the polarizability expression for an exact state. We find that this computationally less demanding approach may show differences up to ˜30 % relative to the excited-state polarizabilities computed using the analytic-derivative formalism.

  13. Dirac spin-orbit torques and charge pumping at the surface of topological insulators

    KAUST Repository

    Ndiaye, Papa B.

    2017-07-07

    We address the nature of spin-orbit torques at the magnetic surfaces of topological insulators using the linear-response theory. We find that the so-called Dirac torques in such systems possess a different symmetry compared to their Rashba counterpart, as well as a high anisotropy as a function of the magnetization direction. In particular, the damping torque vanishes when the magnetization lies in the plane of the topological-insulator surface. We also show that the Onsager reciprocal of the spin-orbit torque, the charge pumping, induces an enhanced anisotropic damping. Via a macrospin model, we numerically demonstrate that these features have important consequences in terms of magnetization switching.

  14. Role of surface gauging in extended particle interactions: The case for spin

    Science.gov (United States)

    Mazilu, Nicolae; Ghizdovat, Vlad; Agop, Maricel

    2016-05-01

    The matter, being extended in space, should be first characterized by a surface of separation from the empty space. This surface cannot be neatly, i.e. purely geometrically, defined. When it comes to extended particles, which thereby are to be considered the fundamental structural units of the matter, the physical evidence points out that they are not even stable: they are in a continuous transformation; and so is their limit of separation from space. The present work describes a concept of extended particle with special emphasis on this limit of separation. It turns out that the properties of inertia, as classically understood, are intrinsically related to the spin properties of quantum origin. Thus, an extended particle model cannot be but "holographic" when it comes to imbedding it in a physical structure. The spin properties turn out to be essential, inasmuch as they decide the forces of interaction issuing from particles.

  15. MONTE CARLO SIMULATION STUDY OF SURFACE ELECTRONIC EXCITATION OF NOBLE METALS

    Institute of Scientific and Technical Information of China (English)

    H.M. Li; Z.J. Ding; Q.R. Pu; Z.M. Zhang

    2002-01-01

    In this work we present a numerical simulation of REELS-spectrum for noble metals,Au and Ag. The calculation is based on an electron-surface inelastic scattering modelpreviously developed. The differential inelastic cross section is obtained fron an inho-mogeneous electron self-energy in the surface region, which provides full informationof the dependency of the total and differential cross section on the kinetic energy,the distance from the surface and the moving direction of electrons, accommodatingthe formulation to the practical situation in surface electron spectroscopes. A novelMonte Carlo simulation code of electron interaction with a surface incorporating thelocal scattering mean free path has been developed. The comparison of the simulatedREELS-spectra with the experimental measurements shows a remarkable agreement onthe spectrum shape, which then confirms that the present model for electron-surfaceinelastic .scattering is quite reasonable. The simulation has further shown the compo.nent to surface excitation due to the individual scattering processes along trajectorypart, i.e., the loss in vacuum before reflection, the loss in vacuum after reflection andloss in metal events.

  16. Spontaneous ferromagnetic spin ordering at the surface of La$_2$CuO$_4$

    OpenAIRE

    2007-01-01

    Magnetic properties of high purity stoichiometric La$_2$CuO$_4$ nanoparticles are systematically investigated as a function of particle size. Ferromagnetic single-domain spin clusters are shown to spontaneously form at the surface of fine grains as well as paramagnetic defects. Hysteresis loops and thermomagnetic irreversibility are observed in a wide temperature range $5 - 350$ K with the remnant moment and coercivity gradually decreasing with increasing temperature. Possible origins of the ...

  17. Magnetic cluster excitations

    Science.gov (United States)

    Furrer, Albert; Waldmann, Oliver

    2013-01-01

    Magnetic clusters, i.e., assemblies of a finite number (between two or three and several hundred) of interacting spin centers which are magnetically decoupled from their environment, can be found in many materials ranging from inorganic compounds and magnetic molecules to artificial metal structures formed on surfaces and metalloproteins. Their magnetic excitation spectra are determined by the nature of the spin centers and of the magnetic interactions, and the particular arrangement of the mutual interaction paths between the spin centers. Small clusters of up to four magnetic ions are ideal model systems in which to examine the fundamental magnetic interactions, which are usually dominated by Heisenberg exchange, but often complemented by anisotropic and/or higher-order interactions. In large magnetic clusters, which may potentially deal with a dozen or more spin centers, there is the possibility of novel many-body quantum states and quantum phenomena. In this review the necessary theoretical concepts and experimental techniques to study the magnetic cluster excitations and the resulting characteristic magnetic properties are introduced, followed by examples of small clusters, demonstrating the enormous amount of detailed physical information that can be retrieved. The current understanding of the excitations and their physical interpretation in the molecular nanomagnets which represent large magnetic clusters is then presented, with a section devoted to the subclass of single-molecule magnets, distinguished by displaying quantum tunneling of the magnetization. Finally, there is a summary of some quantum many-body states which evolve in magnetic insulators characterized by built-in or field-induced magnetic clusters. The review concludes by addressing future perspectives in the field of magnetic cluster excitations.

  18. New high-spin level schemes and excitation modes of {sup 117,118,119,120,122}Cd

    Energy Technology Data Exchange (ETDEWEB)

    Luo, Y.X. [Physics Department, Vanderbilt University, Nashville, TN 37235 (United States); Lawrence Berkeley National Laboratory, Berkeley, CA 94720 (United States); Rasmussen, J.O., E-mail: jorasmussen@lbl.gov [Lawrence Berkeley National Laboratory, Berkeley, CA 94720 (United States); Department of Chemistry, U.C. Berkeley, Berkeley, CA 94720 (United States); Nelson, C.S.; Hamilton, J.H.; Ramayya, A.V.; Hwang, J.K. [Physics Department, Vanderbilt University, Nashville, TN 37235 (United States); Liu, S.H. [Physics Department, Vanderbilt University, Nashville, TN 37235 (United States); Joint Institute for Heavy Ion Research, Oak Ridge, TN 37831 (United States); Goodin, C. [Physics Department, Vanderbilt University, Nashville, TN 37235 (United States); Stone, N.J. [Department of Physics, Oxford University, Oxford OX1 3PU (United Kingdom); Department of Physics and Astronomy, University of Tennessee, Knoxville, TN 37996 (United States); Zhu, S.J. [Physics Department, Vanderbilt University, Nashville, TN 37235 (United States); Department of Physics, Tsinghua University, Beijing 100084 (China); Brewer, N.T.; Li Ke [Physics Department, Vanderbilt University, Nashville, TN 37235 (United States); Lee, I.Y. [Lawrence Berkeley National Laboratory, Berkeley, CA 94720 (United States); Ter-Akopian, G.M. [Flerov Laboratory for Nuclear Reactions, JINR, Dubna (Russian Federation); Daniel, A.V. [Physics Dept., Vanderbilt University, Nashville, TN 37235 (United States); Flerov Laboratory for Nuclear Reactions, JINR, Dubna (Russian Federation); Joint Inst. for Heavy Ion Research, Oak Ridge, TN 37831 (United States); Stoyer, M.A. [Lawrence Livermore National Lab., Livermore, CA 94550 (United States); Donangelo, R. [Facultad de Ingenieria, C.C.30, 11300 Montevideo (Uruguay); Ma, W.C. [Mississippi State Univ., Drawer 5167, Mississippi State, MS 39762 (United States); Cole, J.D. [Idaho National Laboratory, Bldg. IRCPL, MS2114, Idaho Falls, ID 83415 (United States)

    2012-01-15

    High-spin level schemes of {sup 117,118,119,120,122}Cd are expanded by analyzing our high-statistics triple- and higher-fold coincidence events of prompt fission {gamma} rays from {sup 252}Cf at Gammasphere. Spin/parity assignments were made based on new {gamma}-{gamma} angular correlation measurements and level systematics in the neighboring isotopes. Stretch-aligned band structures observed in low-lying levels in {sup 117,119,121}Cd are seen to weaken with increasing spins, with a quasi-rotational degree of freedom manifested at higher spins. The 5{sup -} levels in even-N{sup 118,120}Cd were tentatively interpreted as candidates of quadrupole-octupole (QOC) coupling. The model-independent spin versus Planck-Constant-Over-Two-Pi {omega} curves for even-N and odd-N Cd isotopes imply quasi-rotational alignment of an h{sub 11/2} neutron pair in the even-N Cd isotopes. The relative energies of the lowest 11/2{sup -}, 9/2{sup -}, 7/2{sup -}, and 15/2{sup -} levels in {sup 117}Cd and {sup 119}Cd suggest triaxial shapes based on Meyer-Ter-Vehn theory for these odd-N Cd nuclei. For the even-N Cd isotopes evidence of triaxiality may also be provided by the Shell Correction version of the Tilted Axis Cranking model (SCTAC).

  19. Transparent, superhydrophobic surfaces from one-step spin coating of hydrophobic nanoparticles.

    Science.gov (United States)

    Xu, Lebo; Karunakaran, Raghuraman G; Guo, Jia; Yang, Shu

    2012-02-01

    We study the nonwettability and transparency from the assembly of fluorosilane modified silica nanoparticles (F-SiO(2) NPs) via one-step spin-coating and dip-coating without any surface postpassivation steps. When spin-coating the hydrophobic NPs (100 nm in diameter) at a concentration ≥ 0.8 wt % in a fluorinated solvent, the surface exhibited superhydrophobicity with an advancing water contact angle greater than 150° and a water droplet (5 μL) roll-off angle less than 5°. In comparison, superhydrophobicity was not achieved by dip-coating the same hydrophobic NPs. Scanning electron microscopy (SEM) and atomic force microscopy (AFM) images revealed that NPs formed a nearly close-packed assembly in the superhydrophobic films, which effectively minimized the exposure of the underlying substrate while offering sufficiently trapped air pockets. In the dip-coated films, however, the surface coverage was rather random and incomplete. Therefore, the underlying substrate was exposed and water was able to impregnate between the NPs, leading to smaller water contact angle and larger water contact angle hysteresis. The spin-coated superhydrophobic film was also highly transparent with greater than 95% transmittance in the visible region. Further, we demonstrated that the one-step coating strategy could be extended to different polymeric substrates, including poly(methyl methacrylate) and polyester fabrics, to achieve superhydrophobicity.

  20. Surface Plasmon Polariton Excitation in Metallic Layer Via Surface Relief Gratings in Photoactive Polymer Studied by the Finite-Difference Time-Domain Method.

    Science.gov (United States)

    Karpinski, Pawel; Miniewicz, Andrzej

    2011-09-01

    We performed numerical investigations of surface plasmon excitation and propagation in structures made of a photochromic polymer layer deposited over a metal surface using the finite-difference time-domain method. We investigated the process of light coupling into surface plasmon polariton excitation using surface relief gratings formed on the top of a polymer layer and compared it with the coupling via rectangular ridges grating made directly in the metal layer. We also performed preliminary studies on the influence of refractive index change of photochromic polymer on surface plasmon polariton propagation conditions.

  1. Grating-Coupling-Based Excitation of Bloch Surface Waves for Lab-on-Fiber Nanoprobes

    CERN Document Server

    Scaravilli, Michele; Cusano, Andrea; Galdi, Vincenzo

    2016-01-01

    In this paper, we investigate for the first time the possibility to excite Bloch surface waves (BSWs) on the tip of single-mode optical fibers. Within this framework, we first demonstrate the possibility to exploit a grating-coupling mechanism for on-tip excitation of BSWs, and highlight the flexibility of the proposed design as well as its intrinsic robustness to unavoidable fabrication tolerances. Subsequently, with a view towards label-free chemical and biological sensing, we present an optimized design to maximize the sensitivity (in terms of wavelength shift) of the arising resonances with respect to changes in the refractive properties of the surrounding environment. Numerical results indicate that the attained sensitivities are in line with those exhibited by state-of-the-art plasmonic nanoprobes, with the key advantage of exhibiting much narrower spectral resonances. This prototype study paves the way for a new class of miniaturized high-performance surface-wave fiber-optic devices for high-resolution...

  2. When are Surface Plasmon Polaritons Excited in the Kretschmann-Raether configuration?

    Energy Technology Data Exchange (ETDEWEB)

    Foley, Jonathan J.; Haratyunyan, Hayk; Rosenmann, Daniel; Divan, Ralu; Wiederrecht, Gary P; Gray, Stephen K.

    2015-04-23

    It is widely believed that the reflection minimum in a Kretschmann-Raether experiment results from direct coupling into surface plasmon polariton modes. Our experimental results provide a surprising discrepancy between the leakage radiation patterns of surface plasmon polaritons (SPPs) launched on a layered gold/germanium film compared to the K-R minimum, clearly challenging this belief. We provide definitive evidence that the reflectance dip in K-R experiments does not correlate with excitation of an SPP mode, but rather corresponds to a particular type of perfectly absorbing (PA) mode. Results from rigorous electrodynamics simulations show that the PA mode can only exist under external driving, whereas the SPP can exist in regions free from direct interaction with the driving field. These simulations show that it is possible to indirectly excite propagating SPPs guided by the reflectance minimum in a K-R experiment, but demonstrate the efficiency can be lower by more than a factor of 3. We find that optimal coupling into the SPP can be guided by the square magnitude of the Fresnel transmission amplitude.

  3. Measurement of spin-flip probabilities for ultracold neutrons interacting with nickel phosphorus coated surfaces

    CERN Document Server

    Tang, Z; Brandt, A; Callahan, N B; Clayton, S M; Currie, S A; Ito, T M; Makela, M; Masuda, Y; Morris, C L; Pattie, R; Ramsey, J C; Salvat, D J; Saunders, A; Young, A R

    2015-01-01

    We report a measurement of the spin-flip probabilities for ultracold neutrons interacting with surfaces coated with nickel phosphorus. For 50 $\\mu$m thick nickel phosphorus coated on stainless steel, the spin-flip probability per bounce was found to be $\\beta_{\\rm NiP\\;on\\;SS} = (3.3^{+1.8}_{-5.6}) \\times 10^{-6}$. For 50 $\\mu$m thick nickel phosphorus coated on aluminum, the spin-flip probability per bounce was found to be $\\beta_{\\rm NiP\\;on\\;Al} = (3.6^{+2.1}_{-5.9}) \\times 10^{-6}$. For the copper guide used as reference, the spin flip probability per bounce was found to be $\\beta_{\\rm Cu} = (6.7^{+5.0}_{-2.5}) \\times 10^{-6}$. Nickel phosphorus coated stainless steel or aluminum provides a solution when UCN guides that have a high Fermi potential and are low-cost, mechanically robust, and non-depolarizing are needed.

  4. Interaction induced staggered spin-orbit order in two-dimensional electron gas

    Energy Technology Data Exchange (ETDEWEB)

    Das, Tanmoy [Los Alamos National Laboratory

    2012-06-05

    Decoupling spin and charge transports in solids is among the many prerequisites for realizing spin electronics, spin caloritronics, and spin-Hall effect. Beyond the conventional method of generating and manipulating spin current via magnetic knob, recent advances have expanded the possibility to optical and electrical method which are controllable both internally and externally. Yet, due to the inevitable presence of charge excitations and electrical polarizibility in these methods, the separation between spin and charge degrees of freedom of electrons remains a challenge. Here we propose and formulate an interaction induced staggered spin-orbit order as a new emergent phase of matter. We show that when some form of inherent spin-splitting via Rashba-type spin-orbit coupling renders two helical Fermi surfaces to become significantly nested, a Fermi surface instability arises. To lift this degeneracy, a spontaneous symmetry breaking spin-orbit density wave develops, causing a surprisingly large quasiparticle gapping with chiral electronic states, with no active charge excitations. Since the staggered spin-orbit order is associated with a condensation energy, quantified by the gap value, destroying such spin-orbit interaction costs sufficiently large perturbation field or temperature or de-phasing time. BiAg2 surface state is shown to be a representative system for realizing such novel spin-orbit interaction with tunable and large strength, and the spin-splitting is decoupled from charge excitations.

  5. Magnetic ordering and spin excitations in Mn(dca) sub 2 (pyz) [dca=N(CN) sub 2 sup - , pyz=pyrazine

    CERN Document Server

    Manson, J L; Argyriou, D N; Bordallo, H N; Lynn, J W; Huang, Q; Feyerherm, R; Loose, A

    2002-01-01

    We have studied the T- and H-dependent magnetism in Mn(dca) sub 2 (pyz) [dca=N(CN) sub 2 sup - , pyz=pyrazine] using neutron-scattering methods. The crystal structure can be viewed as a molecular analog of ReO sub 3 , where 1D Mn-pyz-Mn chains connect 2D Mn(dca) sub 2 square sheets to form a 3D network. In zero field, the Mn sup 2 sup + moments order antiferromagnetically below 2.53(2) K along the ac diagonal with a magnitude of 4.15(6) mu B at 1.35 K. The field-dependent response of the [111] magnetic reflection is consistent with spin-flop and induced ferromagnetic phase transitions as previously observed in magnetization measurements. Diffuse-scattering studies indicated no evidence for low-dimensional spin correlations. Using quasielastic neutron scattering, a low-energy spin-wave excitation was observed at propor to 0.23 meV, which is propor to 1/6 the momentum transfer observed in Mn(dca) sub 2 owing to a reduced number of magnetic nearest neighbors. (orig.)

  6. Spontaneous ferromagnetic spin ordering at the surface of La2CuO4

    Science.gov (United States)

    Yusupov, R. V.; Kabanov, V. V.; Mihailovic, D.; Conder, K.; Müller, K. A.; Keller, H.

    2007-07-01

    Magnetic properties of high purity stoichiometric La2CuO4 nanoparticles are systematically investigated as a function of particle size. Ferromagnetic single-domain spin clusters are shown to spontaneously form at the surface of fine grains as well as paramagnetic defects. Hysteresis loops and thermomagnetic irreversibility are observed in a wide temperature range 5-350K with the remnant moment and coercivity gradually decreasing with increasing temperature. Possible origins of the spontaneous surface ferromagnetic clusters and the relation of our data to the appearance of unusual magnetic phenomena and phase separation of doped cuprates are discussed.

  7. Interfacing ion-exchanged waveguide for the efficient excitation of surface plasmons (Presentation Recording)

    Science.gov (United States)

    Beltran Madrigal, Josslyn; Berthel, Martin; Gardillou, Florent; Tellez Limon, Ricardo; Couteau, Christophe; Barbier, Denis; Drezet, Aurelien; Salas-Montiel, Rafael; Huant, Serge; Blaize, Sylvain

    2015-09-01

    Several works have already shown that the excitation of plasmonic structures through waveguides enables a strong light confinement and low propagation losses [1]. This kind of excitation is currently exploited in areas such as biosensing [2], nanocircuits[3] and spectroscopy[4]. Efficient excitation of surface plasmon modes (SPP) with guided modes supported by high-index-contrast waveguides, such as silicon-on-insulator waveguides, had already been shown [1,5], however, the use of weak-confined guided modes of an ion exchanged waveguide on glass as a source of excitation of SPP represents a scientific and technological breakthrough. This is because the integration of plasmonic structures into low-index-contrast waveguide increases the bandwidth of operation and compatibility with conventional optical fibers. In this work, we describe how an adiabatic tapered coupler formed by an intermediate high-index-contrast layer placed between a plasmonic structure and an ion-exchanged waveguide decreases the mismatch between effective indices, size, and shape of the guided modes. This hybrid structure concentrates the electromagnetic energy from the micrometer to the nanometer scale with low coupling losses to radiative modes. The electromagnetic mode confined to the high-index-contrast waveguide then works as an efficient source of SPP supported by metallic nanostructures placed on its surface. We theoretically studied the modal properties and field distribution along the adiabatic coupler structure. In addition, we fabricated a high-index-contrast waveguide by electron beam lithography and thermal evaporation on top of an ion-exchanged waveguide on glass. This structure was characterized with the use of near field scanning optical microscopy (NSOM). Numerical simulations were compared with the experimental results. [1] N. Djaker, R. Hostein, E. Devaux, T. W. Ebbesen, and H. Rigneault, and J. Wenger, J. Phys. Chem. C 114, 16250 (2010). [2] P. Debackere, S. Scheerlinck, P

  8. Technical Note: Reducing the spin-up time of integrated surface water–groundwater models

    KAUST Repository

    Ajami, H.

    2014-12-12

    One of the main challenges in the application of coupled or integrated hydrologic models is specifying a catchment\\'s initial conditions in terms of soil moisture and depth-to-water table (DTWT) distributions. One approach to reducing uncertainty in model initialization is to run the model recursively using either a single year or multiple years of forcing data until the system equilibrates with respect to state and diagnostic variables. However, such "spin-up" approaches often require many years of simulations, making them computationally intensive. In this study, a new hybrid approach was developed to reduce the computational burden of the spin-up procedure by using a combination of model simulations and an empirical DTWT function. The methodology is examined across two distinct catchments located in a temperate region of Denmark and a semi-arid region of Australia. Our results illustrate that the hybrid approach reduced the spin-up period required for an integrated groundwater–surface water–land surface model (ParFlow.CLM) by up to 50%. To generalize results to different climate and catchment conditions, we outline a methodology that is applicable to other coupled or integrated modeling frameworks when initialization from an equilibrium state is required.

  9. Technical Note: Reducing the spin-up time of integrated surface water–groundwater models

    KAUST Repository

    Ajami, H.

    2014-06-26

    One of the main challenges in catchment scale application of coupled/integrated hydrologic models is specifying a catchment\\'s initial conditions in terms of soil moisture and depth to water table (DTWT) distributions. One approach to reduce uncertainty in model initialization is to run the model recursively using a single or multiple years of forcing data until the system equilibrates with respect to state and diagnostic variables. However, such "spin-up" approaches often require many years of simulations, making them computationally intensive. In this study, a new hybrid approach was developed to reduce the computational burden of spin-up time for an integrated groundwater-surface water-land surface model (ParFlow.CLM) by using a combination of ParFlow.CLM simulations and an empirical DTWT function. The methodology is examined in two catchments located in the temperate and semi-arid regions of Denmark and Australia respectively. Our results illustrate that the hybrid approach reduced the spin-up time required by ParFlow.CLM by up to 50%, and we outline a methodology that is applicable to other coupled/integrated modelling frameworks when initialization from equilibrium state is required.

  10. Technical Note: Reducing the spin-up time of integrated surface water–groundwater models

    Directory of Open Access Journals (Sweden)

    H. Ajami

    2014-06-01

    Full Text Available One of the main challenges in catchment scale application of coupled/integrated hydrologic models is specifying a catchment's initial conditions in terms of soil moisture and depth to water table (DTWT distributions. One approach to reduce uncertainty in model initialization is to run the model recursively using a single or multiple years of forcing data until the system equilibrates with respect to state and diagnostic variables. However, such "spin-up" approaches often require many years of simulations, making them computationally intensive. In this study, a new hybrid approach was developed to reduce the computational burden of spin-up time for an integrated groundwater-surface water-land surface model (ParFlow.CLM by using a combination of ParFlow.CLM simulations and an empirical DTWT function. The methodology is examined in two catchments located in the temperate and semi-arid regions of Denmark and Australia respectively. Our results illustrate that the hybrid approach reduced the spin-up time required by ParFlow.CLM by up to 50%, and we outline a methodology that is applicable to other coupled/integrated modelling frameworks when initialization from equilibrium state is required.

  11. Spectroscopic determination of ground and excited state vibrational potential energy surfaces

    Science.gov (United States)

    Laane, Jaan

    Far-infrared spectra, mid-infrared combination band spectra, Raman spectra, and dispersed fluorescence spectra of non-rigid molecules can be used to determine the energies of many of the quantum states of conformationally important vibrations such as out-of-plane ring modes, internal rotations, and molecular inversions in their ground electronic states. Similarly, the fluorescence excitation spectra of jet-cooled molecules, together with electronic absorption spectra, provide the information for determining the vibronic energy levels of electronic excited states. One- or two-dimensional potential energy functions, which govern the conformational changes along the vibrational coordinates, can be determined from these types of data for selected molecules. From these functions the molecular structures, the relative energies between different conformations, the barriers to molecular interconversions, and the forces responsible for the structures can be ascertained. This review describes the experimental and theoretical methodology for carrying out the potential energy determinations and presents a summary of work that has been carried out for both electronic ground and excited states. The results for the out-of-plane ring motions of four-, five-, and six-membered rings will be presented, and results for several molecules with unusual properties will be cited. Potential energy functions for the carbonyl wagging and ring modes for several cyclic ketones in their S1(n,pi*) states will also be discussed. Potential energy surfaces for the three internal rotations, including the one governing the photoisomerization process, will be examined for trans-stilbene in both its S0 and S1(pi,pi*) states. For the bicyclic molecules in the indan family, the two-dimensional potential energy surfaces for the highly interacting ring-puckering and ring-flapping motions in both the S0 and S1(pi,pi*) states have also been determined using all of the spectroscopic methods mentioned above

  12. Slide-free histology via MUSE: UV surface excitation microscopy for imaging unsectioned tissue (Conference Presentation)

    Science.gov (United States)

    Levenson, Richard M.; Harmany, Zachary; Demos, Stavros G.; Fereidouni, Farzad

    2016-03-01

    Widely used methods for preparing and viewing tissue specimens at microscopic resolution have not changed for over a century. They provide high-quality images but can involve time-frames of hours or even weeks, depending on logistics. There is increasing interest in slide-free methods for rapid tissue analysis that can both decrease turn-around times and reduce costs. One new approach is MUSE (microscopy with UV surface excitation), which exploits the shallow penetration of UV light to excite fluorescent signals from only the most superficial tissue elements. The method is non-destructive, and eliminates requirement for conventional histology processing, formalin fixation, paraffin embedding, or thin sectioning. It requires no lasers, confocal, multiphoton or optical coherence tomography optics. MUSE generates diagnostic-quality histological images that can be rendered to resemble conventional hematoxylin- and eosin-stained samples, with enhanced topographical information, from fresh or fixed, but unsectioned tissue, rapidly, with high resolution, simply and inexpensively. We anticipate that there could be widespread adoption in research facilities, hospital-based and stand-alone clinical settings, in local or regional pathology labs, as well as in low-resource environments.

  13. Ozone kinetics in low-pressure discharges: vibrationally excited ozone and molecule formation on surfaces

    Science.gov (United States)

    Marinov, Daniil; Guerra, Vasco; Guaitella, Olivier; Booth, Jean-Paul; Rousseau, Antoine

    2013-10-01

    A combined experimental and modeling investigation of the ozone kinetics in the afterglow of pulsed direct current discharges in oxygen is carried out. The discharge is generated in a cylindrical silica tube of radius 1 cm, with short pulse durations between 0.5 and 2 ms, pressures in the range 1-5 Torr and discharge currents ˜40-120 mA. Time-resolved absolute concentrations of ground-state atoms and ozone molecules were measured simultaneously in situ, by two-photon absorption laser-induced fluorescence and ultraviolet absorption, respectively. The experiments were complemented by a self-consistent model developed to interpret the results and, in particular, to evaluate the roles of vibrationally excited ozone and of ozone formation on surfaces. It is found that vibrationally excited ozone, O_3^{*} , plays an important role in the ozone kinetics, leading to a decrease in the ozone concentration and an increase in its formation time. In turn, the kinetics of O_3^{*} is strongly coupled with those of atomic oxygen and O2(a 1Δg) metastables. Ozone formation at the wall does not contribute significantly to the total ozone production under the present conditions. Upper limits for the effective heterogeneous recombination probability of O atoms into ozone are established.

  14. Investigation of laser-surface interactions and optical damage mechanisms using excitation by pairs of picosecond laser pulses

    Science.gov (United States)

    Chase, L. L.; Lee, H. W. H.; Hughes, Robert S.

    1990-07-01

    It is demonstrated that laser-surface interactions that cause optical surface damage of nominally transparent materials can be investigated by observing the effects of excitation by pairs of picosecond pulses separated by a variable time delay. Laser-induced emission of neutrals is used as the detection mechanism in the present experiments.

  15. NMR investigations of surfaces and interfaces using spin-polarized xenon

    Energy Technology Data Exchange (ETDEWEB)

    Gaede, Holly Caroline [Univ. of California, Berkeley, CA (United States). Dept. of Chemistry

    1995-07-01

    129Xe NMR is potentially useful for the investigation of material surfaces, but has been limited to high surface area samples in which sufficient xenon can be loaded to achieve acceptable signal to noise ratios. In Chapter 2 conventional 129Xe NMR is used to study a high surface area polymer, a catalyst, and a confined liquid crystal to determine the topology of these systems. Further information about the spatial proximity of different sites of the catalyst and liquid crystal systems is determined through two dimensional exchange NMR in Chapter 3. Lower surface area systems may be investigated with spin-polarized xenon, which may be achieved through optical pumping and spin exchange. Optically polarized xenon can be up to 105times more sensitive than thermally polarized xenon. In Chapter 4 highly polarized xenon is used to examine the surface of poly(acrylonitrile) and the formation of xenon clathrate hydrates. An attractive use of polarized xenon is as a magnetization source in cross polarization experiments. Cross polarization from adsorbed polarized xenon may allow detection of surface nuclei with drastic enhancements. A non-selective low field thermal mixing technique is used to enhance the 13C signal of CO2 of xenon occluded in solid CO2 by a factor of 200. High-field cross polarization from xenon to proton on the surface of high surface area polymers has enabled signal enhancements of ~1,000. These studies, together with investigations of the efficiency of the cross polarization process from polarized xenon, are discussed in Chapter 5. Another use of polarized xenon is as an imaging contrast agent in systems that are not compatible with traditional contrast agents. The resolution attainable with this method is determined through images of structured phantoms in Chapter 6.

  16. Constructing a superhydrophobic surface on polydimethylsiloxane via spin coating and vapor-liquid sol-gel process.

    Science.gov (United States)

    Peng, Yu-Ting; Lo, Kuo-Feng; Juang, Yi-Je

    2010-04-06

    In this study, a superhydrophobic surface on polydimethylsiloxane (PDMS) substrate was constructed via the proposed vapor-liquid sol-gel process in conjunction with spin coating of dodecyltrichlorosilane (DTS). Unlike the conventional sol-gel process where the reaction takes place in the liquid phase, layers of silica (SiO(2)) particles were formed through the reaction between the reactant spin-coated on the PDMS surface and vapor of the acid solution. This led to the SiO(2) particles inlaid on the PDMS surface. Followed by subsequent spin coating of DTS solution, the wrinkle-like structure was formed, and the static contact angle of the water droplet on the surface could reach 162 degrees with 2 degrees sliding angle and less than 5 degrees contact angle hysteresis. The effect of layers of SiO(2) particles, concentrations of DTS solution and surface topography on superhydrophobicity of the surface is discussed.

  17. Surface spin-polarized currents generated in topological insulators by circularly polarized synchrotron radiation and their photoelectron spectroscopy indication

    Science.gov (United States)

    Shikin, A. M.; Klimovskikh, I. I.; Filyanina, M. V.; Rybkina, A. A.; Pudikov, D. A.; Kokh, K. A.; Tereshchenko, O. E.

    2016-08-01

    A new method for generating spin-polarized currents in topological insulators has been proposed and investigated. The method is associated with the spin-dependent asymmetry of the generation of holes at the Fermi level for branches of topological surface states with the opposite spin orientation under the circularly polarized synchrotron radiation. The result of the generation of holes is the formation of compensating spin-polarized currents, the value of which is determined by the concentration of the generated holes and depends on the specific features of the electronic and spin structures of the system. The indicator of the formed spin-polarized current can be a shift of the Fermi edge in the photoelectron spectra upon photoexcitation by synchrotron radiation with the opposite circular polarization. The topological insulators with different stoichiometric compositions (Bi1.5Sb0.5Te1.8Se1.2 and PbBi2Se2Te2) have been investigated. It has been found that there is a correlation in the shifts and generated spin-polarized currents with the specific features of the electronic spin structure. Investigations of the graphene/Pt(111) system have demonstrated the possibility of using this method for other systems with a spin-polarized electronic structure.

  18. Oblique-incidence excitation of surface plasmon polaritons on small metal wires

    CERN Document Server

    Kriesch, Arian

    2008-08-13

    This work reports on the experimental investigation of surface plasmon polaritons (SPP) on cylindrical wires of small diameters. Applying a new technique that was developed by this group and recently reported, single wire and wire array samples of gold (Au) and silver (Ag) with small diameters 400nm < D < 3 mum and high aspect ratios <= 75000 in photonic crystal fibers and single hole capillaries are fabricated. Additionally, effective bulk metal wires of Au and Ag are created by a hybrid technique, including fiber tapering and magnetron sputter deposition for a large number of different diameters between 13 mum to 50 mum. The measurement of the absorption, corresponding to the excitation of SPP modes is realized with a new goniometer-based experimental setup for oblique incidence laser beam scattering at a single wavelength. A device is developed that allows a simultaneous measurement of the scattering amplitude in s- and p-polarization under varied incident angle. For comparison, a model for the di...

  19. Unidirectional transmission based on polarization conversion and excitation of magnetic or surface polaritons

    Science.gov (United States)

    Wu, Xiaohu; Fu, Ceji

    2017-07-01

    We propose in this work combing a uniaxial crystal slab with a one-dimensional grating to realize unidirectional transmission (UDT). The physical mechanism for the UDT is attributed to polarization conversion with uniaxial crystal slab and excitation of magnetic polaritons (MPs) or surface plasmon polaritons (SPPs) in the grating region. Numerical simulations were performed by taking hexagonal boron nitride as the uniaxial crystal. The results reveal that UDT can be achieved for both TE and TM waves in the mid-infrared and the optical regions if the grating material is respectively selected as silicon carbide (SiC) and silver (Ag) with properly chosen values of the structure's geometric parameters. This work may provide important guidelines for design of novel unidirectional transmission devices.

  20. Unidirectional transmission based on polarization conversion and excitation of magnetic or surface polaritons

    Directory of Open Access Journals (Sweden)

    Xiaohu Wu

    2017-07-01

    Full Text Available We propose in this work combing a uniaxial crystal slab with a one-dimensional grating to realize unidirectional transmission (UDT. The physical mechanism for the UDT is attributed to polarization conversion with uniaxial crystal slab and excitation of magnetic polaritons (MPs or surface plasmon polaritons (SPPs in the grating region. Numerical simulations were performed by taking hexagonal boron nitride as the uniaxial crystal. The results reveal that UDT can be achieved for both TE and TM waves in the mid-infrared and the optical regions if the grating material is respectively selected as silicon carbide (SiC and silver (Ag with properly chosen values of the structure’s geometric parameters. This work may provide important guidelines for design of novel unidirectional transmission devices.

  1. Photoluminescence from single silicon quantum dots excited via surface plasmon polaritons

    Energy Technology Data Exchange (ETDEWEB)

    Matsuhisa, Koji [Department of Electrical and Electronic Engineering, Graduate School of Engineering, Kobe University, Rokkodai, Nada, Kobe 657-8501 (Japan); Fujii, Minoru, E-mail: fujii@eedept.kobe-u.ac.jp [Department of Electrical and Electronic Engineering, Graduate School of Engineering, Kobe University, Rokkodai, Nada, Kobe 657-8501 (Japan); Imakita, Kenji; Hayashi, Shinji [Department of Electrical and Electronic Engineering, Graduate School of Engineering, Kobe University, Rokkodai, Nada, Kobe 657-8501 (Japan)

    2012-05-15

    Single dot spectroscopy of Si quantum dots (QDs) was performed by using surface plasmon polariton (SPP)-mediated excitation in the attenuated total reflection geometry with a MgF{sub 2}/Ag film on the base of a prism. Thanks to the 16 times enhancement of the incident electric field and very small background signal, PL from single Si QDs was observed clearly. This proves the usefulness of the technique for the detection of inherently weak emission of Si QDs. - Highlights: Black-Right-Pointing-Pointer Metal-enhanced fluorescence for the single dot spectroscopy of Si QDs. Black-Right-Pointing-Pointer Single dot spectroscopy of Si QDs in the attenuated total reflection geometry. Black-Right-Pointing-Pointer Single Si QDs prepared from silica films containing Si QDs.

  2. Spin glasses

    CERN Document Server

    Bovier, Anton

    2007-01-01

    Spin glass theory is going through a stunning period of progress while finding exciting new applications in areas beyond theoretical physics, in particular in combinatorics and computer science. This collection of state-of-the-art review papers written by leading experts in the field covers the topic from a wide variety of angles. The topics covered are mean field spin glasses, including a pedagogical account of Talagrand's proof of the Parisi solution, short range spin glasses, emphasizing the open problem of the relevance of the mean-field theory for lattice models, and the dynamics of spin glasses, in particular the problem of ageing in mean field models. The book will serve as a concise introduction to the state of the art of spin glass theory, usefull to both graduate students and young researchers, as well as to anyone curious to know what is going on in this exciting area of mathematical physics.

  3. "Click-functional" block copolymers provide precise surface functionality via spin coating.

    Science.gov (United States)

    Rengifo, Hernán R; Chen, Lu; Grigoras, Cristian; Ju, Jingyue; Koberstein, Jeffrey T

    2008-07-15

    There are few existing methods for the quantitative functionalization of surfaces, especially for polymeric substrates. We demonstrate that alkyne end-functional diblock copolymers can be used to provide precise areal densities of reactive functionality on both hard (e.g., glass and silicon oxide) and soft (i.e., polymeric) substrates. Alkyne functionality is extremely versatile because the resultant functional surfaces are reactive toward azide functional molecules by Sharpless click chemistry. Spin-coated films of alpha-alkyne-omega-Br-poly( tert-butylacrylate- b-methylmethacrylate) (poly( tBA-MMA)) spontaneously self-assemble on the aforementioned substrates to present a surface monolayer of PtBA with a thickness in the range of 1 to 9 nm. The PMMA block physisorbs to provide multivalent anchoring onto hard substrates and is fixed onto polymer surfaces by interpenetration with the substrate polymer. The areal density of alkyne functional groups is precisely controlled by adjusting the thickness of the block copolymer monolayer, which is accomplished by changing either the spin coating conditions (i.e., rotational speed and solution concentration) or the copolymer molecular weight. The reactivity of surface-bound alkynes, in 1,3-dipolar cycloaddition reactions or by so-called "click chemistry", is demonstrated by covalent surface immobilization of fluorescently labeled azides. The modificed surfaces are characterized by atomic force microscopy (AFM), contact angle, ellipsometry, fluorescent imaging and angle-dependent X-ray photoelectron spectroscopy (ADXPS) measurements. Microarrays of covalently bound fluorescent molecules are created to demonstrate the approach and their performance is evaluated by determining their fluorescence signal-to-noise ratios.

  4. The study of quasi-projectiles produced in Ni+Ni and Ni+Au collisions: excitation energy and spin; Etude des quasi-projectiles produits dans les collisions Ni+Ni et Ni+Au: energie d'excitation et spin

    Energy Technology Data Exchange (ETDEWEB)

    Buta, A

    2003-02-01

    During the collision between the projectile and the target nuclei in the intermediate energy regime (E < 100 MeV/nucleon) two excited nuclei are mainly observed in the exit channel, the quasi projectile (QP) and the quasi target. They disintegrate by particle emission. However, this binary picture is perturbed by the emission of particles and light fragments with velocities intermediate between the projectile velocity and the target one, all along the interaction (midrapidity component). This work aim to determine the excitation energy and the intrinsic angular momentum (or spin) of quasi-projectiles produced in the Ni+Ni and Ni+Au collisions at 52 and 90 MeV/nucleon. The excitation energy is deduced from the kinematical characteristics of particles emitted by the quasi-projectile. They have to be separated from midrapidity particles. Three different scenarios have been used for this purpose. The spin of the quasi-projectile has been extracted from the experimental data by mean of proton and alpha particles multiplicities emitted by the QP in the Ni+Au at 52 MeV/nucleon reaction. The results have been compared to the predictions of a theoretical model based on nucleon transfers. Their evolution is qualitatively reproduced as a function of the violence of the collision. (author)

  5. Engineering electrocatalytic activity in nanosized perovskite cobaltite through surface spin-state transition

    Science.gov (United States)

    Zhou, Shiming; Miao, Xianbing; Zhao, Xu; Ma, Chao; Qiu, Yuhao; Hu, Zhenpeng; Zhao, Jiyin; Shi, Lei; Zeng, Jie

    2016-05-01

    The activity of electrocatalysts exhibits a strongly dependence on their electronic structures. Specifically, for perovskite oxides, Shao-Horn and co-workers have reported a correlation between the oxygen evolution reaction activity and the eg orbital occupation of transition-metal ions, which provides guidelines for the design of highly active catalysts. Here we demonstrate a facile method to engineer the eg filling of perovskite cobaltite LaCoO3 for improving the oxygen evolution reaction activity. By reducing the particle size to ~80 nm, the eg filling of cobalt ions is successfully increased from unity to near the optimal configuration of 1.2 expected by Shao-Horn's principle. Consequently, the activity is significantly enhanced, comparable to those of recently reported cobalt oxides with eg~1.2 configurations. This enhancement is ascribed to the emergence of spin-state transition from low-spin to high-spin states for cobalt ions at the surface of the nanoparticles, leading to more active sites with increased reactivity.

  6. Electrochemical immobilization of Fluorescent labelled probe molecules on a FTO surface for affinity detection based on photo-excited current

    Energy Technology Data Exchange (ETDEWEB)

    Haruyama, Tetsuya; Wakabayashi, Ryo; Cho, Takeshi; Matsuyama, Sho-taro, E-mail: haruyama@life.kyutech.as.jp [Kyushu Institute of Technology, Department of Biological Functions and Engineering, Kitakyushu Science and Research Park, Hibikino, Kitakyushu, Fukuoka 808-0196 (Japan)

    2011-10-29

    Photo-excited current can be generated at a molecular interface between a photo-excited molecules and a semi-conductive material in appropriate condition. The system has been recognized for promoting photo-energy devices such as an organic dye sensitized solar-cell. The photo-current generated reactions are totally dependent on the interfacial energy reactions, which are in a highly fluctuated interfacial environment. The authors investigated the photo-excited current reaction to develop a smart affinity detection method. However, in order to perform both an affinity reaction and a photo-excited current reaction at a molecular interface, ordered fabrications of the functional (affinity, photo-excitation, etc.) molecules layer on a semi-conductive surface is required. In the present research, we would like to present the fabrication and functional performance of photo-excited current-based affinity assay device and its application for detection of endocrine disrupting chemicals. On the FTO surface, fluorescent pigment labelled affinity peptide was immobilized through the EC tag (electrochemical-tag) method. The modified FTO produced a current when it was irradiated with diode laser light. However, the photo current decreased drastically when estrogen (ES) coexisted in the reaction solution. In this case, immobilized affinity probe molecules formed a complex with ES and estrogen receptor (ER). The result strongly suggests that the photo-excited current transduction between probe molecule-labelled cyanine pigment and the FTO surface was partly inhibited by a complex that formed at the affinity oligo-peptide region in a probe molecule on the FTO electrode. The bound bulky complex may act as an impediment to perform smooth transduction of photo-excited current in the molecular interface. The present system is new type of photo-reaction-based analysis. This system can be used to perform simple high-sensitive homogeneous assays.

  7. Integrable generalizations of Schrodinger maps and Heisenberg spin models from Hamiltonian flows of curves and surfaces

    CERN Document Server

    Anco, S C

    2010-01-01

    A moving frame formulation of non-stretching geometric curve flows in Euclidean space is used to derive a 1+1 dimensional hierarchy of integrable SO(3)-invariant vector models containing the Heisenberg ferromagnetic spin model as well as a model given by a spin-vector version of the mKdV equation. These models describe a geometric realization of the NLS hierarchy of soliton equations whose bi-Hamiltonian structure is shown to be encoded in the Frenet equations of the moving frame. This derivation yields an explicit bi-Hamiltonian structure, recursion operator, and constants of motion for each model in the hierarchy. A generalization of these results to geometric surface flows is presented, where the surfaces are non-stretching in one direction while stretching in all transverse directions. Through the Frenet equations of a moving frame, such surface flows are shown to encode a hierarchy of 2+1 dimensional integrable SO(3)-invariant vector models, along with their bi-Hamiltonian structure, recursion operator, ...

  8. Relationship of magnetic behavior and surface spin coupling in Hematite nanowires bundles

    Science.gov (United States)

    Li, D. P.; Zhang, Y.; Wang, P. F.; Xu, J. C.; Han, Y. B.; Jin, H. X.; Jin, D. F.; Peng, X. L.; Hong, B.; Li, J.; Yang, Y. T.; Gong, J.; Ge, H. L.; Wang, X. Q.

    2016-08-01

    Hematite (α-Fe2O3) nanowires were synthesized using mesoporous SBA-15 silica as the hard templates, and then the well-dispersed α-Fe2O3 nanowires (NWS) were separated from the ordered α-Fe2O3 nanowires bundles (NWBS) by the centrifugation technique. X-ray diffraction (XRD), transmission electron microscopy (TEM) and surperconducting quantum interference device (SQUID) were used to characterize the microstructure and magnetic properties of the as-prepared samples. All results indicated that the α-Fe2O3 NWS and NWBS with the different interwires distance presented the same diameter for nanowires, which was possible to reveal the exchange interaction between α-Fe2O3 NWBs. Both samples showed ferromagnetism and α-Fe2O3 NWS presented superparamagnetism at high temperature. The magnetic results indicated the surface spin between the neighboring nanowires of α-Fe2O3 NWBs coupled each other. The saturation magnetization of α-Fe2O3 NWBS was lower than that of α-Fe2O3 NWS, while the coercivity and Curie temperature were larger. It was concluded that the surface spin coupling could weaken the surface effect on the magnetic properties for nanostructures.

  9. Density-of-state oscillation of quasiparticle excitation in the spin density wave phase of (TMTSF)2ClO4.

    Science.gov (United States)

    Uji, S; Kimata, M; Moriyama, S; Yamada, J; Graf, D; Brooks, J S

    2010-12-31

    Systematic measurements of the magnetocaloric effect, heat capacity, and magnetic torque under a high magnetic field up to 35 T are performed in the spin density wave (SDW) phase of a quasi-one-dimensional organic conductor (TMTSF)2ClO4. In the SDW phase above 26 T, where the quantum Hall effect is broken, rapid oscillations (ROs) in these thermodynamic quantities are observed, which provides clear evidence of the density-of-state (DOS) oscillation near the Fermi level. The resistance is semiconducting and the heat capacity divided by temperature is extrapolated to zero at 0 K in the SDW phase, showing that all the energy bands are gapped, and there is no DOS at the Fermi level. The results show that the ROs are ascribed to the DOS oscillation of the quasiparticle excitation.

  10. Collective spin-excitations in Cu L and O K edge resonant inelastic X-ray scattering from Sr{sub 14}Cu{sub 24}O{sub 41}

    Energy Technology Data Exchange (ETDEWEB)

    Schmitt, Thorsten; Schlappa, Justina; Vernay, F.; Strocov, V.; Thielemann, B.; Ronnow, H.; Mesot, J.; Delley, B.; Patthey, L. [Paul Scherrer Institut, Villigen PSI (Switzerland); Ilakovac, V. [UPMC, Paris (France)

    2009-07-01

    The spin-ladder/spin-chain compound Sr{sub 14}Cu{sub 24}O{sub 41} is a low-dimensional spin system, which is known for its complex interplay between charge and spin degrees of freedom. One of the subsystems is formed by 2-leg ladders Cu{sub 2}O{sub 3}, which have the properties of a spin liquid with a finite spin gap. Resonant inelastic X-ray scattering (RIXS) is a powerful probe of the electronic ground state and the low-energy excitation spectrum of transition-metal oxides, being directly sensitive to the valence electron configuration. Using RIXS at the Cu L{sub 3} and O K edge of Sr{sub 14}Cu{sub 24}O{sub 41} we observe collective spin-excitations from the ladders, which we assign to two-triplon modes. At the Cu L{sub 3} resonance the dispersion of the modes was mapped out depending on the momentum transfer with excellent sensitivity over almost the entire first Brillouin-zone, in contrast to inelastic neutron scattering. Site-sensitive RIXS at the O K edge of the chain- and ladder-subsystems give insight into the character of the holes.

  11. Organic semiconductors: What makes the spin relax?

    Science.gov (United States)

    Bobbert, Peter A.

    2010-04-01

    Spin relaxation in organic materials is expected to be slow because of weak spin-orbit coupling. The effects of deuteration and coherent spin excitation show that the spin-relaxation time is actually limited by hyperfine fields.

  12. Theoretical study on the low-lying excited states of the phosphorus monoiodide (PI) including the spin-orbit coupling

    Science.gov (United States)

    Zhang, Xiaomei; Liu, Xiaoting; Liang, Guiying; Li, Rui; Xu, Haifeng; Yan, Bing

    2016-01-01

    The potential energy curves (PECs) of the 22 Λ-S states of the phosphorus monoiodide (PI) molecule have been calculated at the level of MRCI+Q method with correlation-consistent quadruple-ζ quality basis set. The spectroscopic constants of the bound states are determined, which well reproduce the available measurements. The metastable a1Δ state has been reported for the first time, which lies between the X3Σ- and b1Σ+ states and have much deeper well than the ground state. The R-dependent spin-orbit (SO) matrix elements are calculated with the full-electron Breit-Pauli operator. Based on the SO matrix elements, the perturbations that the 23Π state may suffer from are analyzed in detail. The SOC effect makes the original Λ-S states split into 51 Ω states. In the zero-field splitting of the ground state X3Σ-, the spin-spin coupling contribution (2.23 cm-1) is found to be much smaller compared to the spin-orbit coupling contribution (50 cm-1). The avoided crossings between the Ω states lead to much shallower potential wells and the change of dissociation relationships of the states. The Ω-state wavefunctions are analyzed depending on their Λ-S compositions, showing the strong interactions among several quasidegenerate Λ-S states of the same total SO symmetry. The transition properties including electric dipole (E1), magnetic dipole (M1), and electric quadrupole (E2) transition moments (TMs), the Franck-Condon factors, the transition probabilities and the radiative lifetimes are computed for the transitions between Ω components of a1Δ and b1Σ+ states and ground state. The transition probabilities induced by the E1, E2, and M1 transitions are evaluated. The E2 makes little effect on transition probabilities. In contrast, the E1 transition makes the main contribution to the transition probability and the M1 transition also brings the influence that cannot be neglected. Finally, the radiative lifetimes are determined with the transition moments including E

  13. Features in Quasi-particle Excitations and Tunnelling Spectra due to Coupling to Spin Fluctuations in High-Tc Cuprates

    Institute of Scientific and Technical Information of China (English)

    赵力; 李建新; 龚昌德; 赵柏儒

    2002-01-01

    In a self-consistent mean-field treatment of the two-dimensional t - t' - J model, we theoretically examine thecoupling of in-plane quasi-particles to the antiferromagnetic spin fluctuations in high-Tc superconductors, whichrenormalizes the fermionic self-energy. We reproduce the characteristic peak,lip-hump structure observed notonly in angle-resolved photoemission spectroscopy, but also in superconductor-insulator-normal metal junctionsand scanning tunnelling microscopy experiments. We consider the evolution of this structure with doping. Itis shown that this kind of coupling can account for many anomalous properties of high-Tc superconductors insuperconducting states.

  14. DQ-DRENAR with back-to-back (BABA) excitation: Measuring homonuclear dipole-dipole interactions in multiple spin-1/2 systems.

    Science.gov (United States)

    Ren, Jinjun; Eckert, Hellmut

    2015-10-01

    A new pulse sequence entitled DQ-DRENAR, (Double-Quantum based Dipolar Recoupling Effects Nuclear Alignment Reduction) was recently described for the quantitative measurement of magnetic dipole-dipole interactions in homonuclear spin-1/2 systems involving multiple nuclei. The double quantum coherences were created via a windowless symmetry-based pulse sequence (POST-C7). The present contribution evaluates the performance of the "Back-to-Back" excitation pulse scheme BABA-xy16 in such DRENAR experiments. Using SIMPSON simulations, special attention is given to finite pulse length effects, dipolar truncation, and chemical shift anisotropy interference. Experimental results on model compounds demonstrate good stability up to long mixing times (>10 ms) as well as high accuracy. As its dipolar coupling efficiency is relatively high (the dipolar coupling scaling factor is 4.24 times as high as that of POST-C7), DQ-DRENAR-BABA-xy16 is most appropriate for the measurement of relatively weak dipolar coupling strengths (<400 Hz). Different from POST-C7, for which the spinning rate is limited to 1/7 of the nutation frequency, DQ-DRENAR-BABA-xy16 experiments can take full advantage of ultrafast MAS experiments.

  15. Excitation of surface plasmon polariton modes with multiple nitrogen vacancy centers in single nanodiamonds

    Science.gov (United States)

    Kumar, Shailesh; Lausen, Jens L.; Garcia-Ortiz, Cesar E.; Andersen, Sebastian K. H.; Roberts, Alexander S.; Radko, Ilya P.; Smith, Cameron L. C.; Kristensen, Anders; Bozhevolnyi, Sergey I.

    2016-02-01

    Nitrogen-vacancy (NV) centers in diamonds are interesting due to their remarkable characteristics that are well suited to applications in quantum-information processing and magnetic field sensing, as well as representing stable fluorescent sources. Multiple NV centers in nanodiamonds (NDs) are especially useful as biological fluorophores due to their chemical neutrality, brightness and room-temperature photostability. Furthermore, NDs containing multiple NV centers also have potential in high-precision magnetic field and temperature sensing. Coupling NV centers to propagating surface plasmon polariton (SPP) modes gives a base for lab-on-a-chip sensing devices, allows enhanced fluorescence emission and collection which can further enhance the precision of NV-based sensors. Here, we investigate coupling of multiple NV centers in individual NDs to the SPP modes supported by silver surfaces protected by thin dielectric layers and by gold V-grooves (VGs) produced via the self-terminated silicon etching. In the first case, we concentrate on monitoring differences in fluorescence spectra obtained from a source ND, which is illuminated by a pump laser, and from a scattering ND illuminated only by the fluorescence-excited SPP radiation. In the second case, we observe changes in the average NV lifetime when the same ND is characterized outside and inside a VG. Fluorescence emission from the VG terminations is also observed, which confirms the NV coupling to the VG-supported SPP modes.

  16. Fundamentally excited flow past a surface-mounted rib. Part I: Turbulent structure characterisation

    Indian Academy of Sciences (India)

    P K Panigrahi

    2001-10-01

    Different data analysis techniques for characterisation of the turbulent flow past a surface-mounted rib are reviewed. Deficiencies of the existing techniques are explained and modified techniques for determination of coherent structure magnitude and phase jitter are suggested. The effect of fundamental excitation on the flow is studied by using these turbulent signal analysis techniques. The appropriate length scale for characterizing the large-scale structures present in the reattaching shear layer of the surface-mounted rib is found to be the momentum thickness at the downstream edge of the rib, and the corresponding Strouhal number is 0.013. This is in contrast to a rib in the free stream, where the rib height is the correct scaling parameter. The post reattachment region is observed to be dominated by large-scale structures contrary to the traditional belief that large eddies break into small scales at the reattachment location. Low magnitude of phase jitter in the near field region is observed, indicating coherence of the flow structures. Phase decorrelation begins to occur beyond three rib heights from the downstream edge of the rib. From the quadrant analysis results, the outer edge of the shear layer is observed to be dominated by large-scale ejection motions.

  17. Excited-state intramolecular proton transfer to carbon atoms: nonadiabatic surface-hopping dynamics simulations.

    Science.gov (United States)

    Xia, Shu-Hua; Xie, Bin-Bin; Fang, Qiu; Cui, Ganglong; Thiel, Walter

    2015-04-21

    Excited-state intramolecular proton transfer (ESIPT) between two highly electronegative atoms, for example, oxygen and nitrogen, has been intensely studied experimentally and computationally, whereas there has been much less theoretical work on ESIPT to other atoms such as carbon. We have employed CASSCF, MS-CASPT2, RI-ADC(2), OM2/MRCI, DFT, and TDDFT methods to study the mechanistic photochemistry of 2-phenylphenol, for which such an ESIPT has been observed experimentally. According to static electronic structure calculations, irradiation of 2-phenylphenol populates the bright S1 state, which has a rather flat potential in the Franck-Condon region (with a shallow enol minimum at the CASSCF level) and may undergo an essentially barrierless ESIPT to the more stable S1 keto species. There are two S1/S0 conical intersections that mediate relaxation to the ground state, one in the enol region and one in the keto region, with the latter one substantially lower in energy. After S1 → S0 internal conversion, the transient keto species can return back to the S0 enol structure via reverse ground-state hydrogen transfer in a facile tautomerization. This mechanistic scenario is verified by OM2/MRCI-based fewest-switches surface-hopping simulations that provide detailed dynamic information. In these trajectories, ESIPT is complete within 118 fs; the corresponding S1 excited-state lifetime is computed to be 373 fs in vacuum. Most of the trajectories decay to the ground state via the S1/S0 conical intersection in the keto region (67%), and the remaining ones via the enol region (33%). The combination of static electronic structure computations and nonadiabatic dynamics simulations is expected to be generally useful for understanding the mechanistic photophysics and photochemistry of molecules with intramolecular hydrogen bonds.

  18. In-plane anisotropy of the spin excitation spectrum in strongly underdoped YBa{sub 2}Cu{sub 3}O{sub 6+x}

    Energy Technology Data Exchange (ETDEWEB)

    Haug, Daniel; Hinkov, Vladimir; Lin, Chengtian; Keimer, Bernhard [Max-Planck-Institut fuer Festkoerperforschung, Stuttgart (Germany); Fauque, Benoit; Bourges, Philippe; Sidis, Yvan [Laboratoire Leon Brillouin, CEA-CNRS Saclay (France); Ivanov, Alexandre [Institut Laue-Langevin, Grenoble (France)

    2008-07-01

    The spin excitation spectrum of the optimally doped and moderately underdoped high-temperature superconductor YBa{sub 2}Cu{sub 3}O{sub 6+x} is dominated by the so-called resonance peak for excitation energies between 30 and 40 meV (depending on the oxygen content x) that sets in abruptly below T{sub c}. Here we report measurements on arrays of untwinned single crystals in the strongly underdoped regime in which the situation is very different: Spectral weight is shifted towards low energies and evolves smoothly through T{sub c}. The spectrum exhibits a peak below {proportional_to}10 meV which shows a spontaneous onset of a strong anisotropy in the a-b-plane defined by the CuO{sub 2} layers. This phenomenon matches the symmetry properties of a nematic liquid crystal, a new symmetry-broken electronic phase that coexists with high-temperature superconductivity in strongly underdoped cuprates.

  19. Two-Dimensional Metallicity with a Large Spin-Orbit Splitting: DFT Calculations of the Atomic, Electronic, and Spin Structures of the Au/Ge(111-(3×3R30° Surface

    Directory of Open Access Journals (Sweden)

    Andrzej Fleszar

    2015-01-01

    of the many-body effects (self-interaction corrections beyond the LDA or GGA approximations. The most interesting property of this surface system is the large spin splitting of its metallic surface bands and the undulating spin texture along the hexagonal Fermi contours, which highly resembles the spin texture at the Dirac state of the topological insulator Bi2Te3. These properties make this system particularly interesting from both fundamental and technological points of view.

  20. Bulk and surface phase transitions in the three-dimensional O(4) spin model

    Science.gov (United States)

    Deng, Youjin

    2006-05-01

    We investigate the O(4) spin model on the simple-cubic lattice by means of the Wolff cluster algorithm. Using the toroidal boundary condition, we locate the bulk critical point at coupling Kc=0.935856(2) , and determine the bulk thermal magnetic renormalization exponents as yt=1.3375(15) and yh=2.4820(2) , respectively. The universal ratio Q=⟨m2⟩2/⟨m4⟩ is also determined as 0.9142(1). The precision of these estimates significantly improves over that of the existing results. Then, we simulate the critical O(4) model with two open surfaces on which the coupling strength K1 can be varied. At the ordinary transitions, the surface magnetic exponent is determined as yh1(o)=1.0202(12) . Further, we find a so-called special surface transition at κ=K1/K-1=1.258(20) . At this point, the surface thermal exponent yt1(s) is rather close to zero, and we cannot exclude that the corresponding surface transition is Kosterlitz-Thouless-like. The surface magnetic exponent is yh1(s)=1.816(2) .

  1. Bulk and surface phase transitions in the three-dimensional O4 spin model.

    Science.gov (United States)

    Deng, Youjin

    2006-05-01

    We investigate the O(4) spin model on the simple-cubic lattice by means of the Wolff cluster algorithm. Using the toroidal boundary condition, we locate the bulk critical point at coupling K(c) = 0.935 856(2), and determine the bulk thermal magnetic renormalization exponents as y(t) = 1.337 5(15) and y(h) = 2.482 0(2), respectively. The universal ratio Q=m(2)(2)/m(4) is also determined as 0.9142(1). The precision of these estimates significantly improves over that of the existing results. Then, we simulate the critical O(4) model with two open surfaces on which the coupling strength K(1) can be varied. At the ordinary transitions, the surface magnetic exponent is determined as y((o))(h1) = 1.020 2(12). Further, we find a so-called special surface transition at (k) = K(1)/K-1 = 1.258(20). At this point, the surface thermal exponent y(s)(t1) is rather close to zero, and we cannot exclude that the corresponding surface transition is Kosterlitz-Thouless-like. The surface magnetic exponent is y((s))/h1 = 1.816(2).

  2. Second harmonic generation in NLO polymers excited by Surface Plasmon enhanced electric field induced by femtosecond optical pulses

    Directory of Open Access Journals (Sweden)

    Kawata Y.

    2013-03-01

    Full Text Available We will report second harmonic generation (SHG in nonlinear optical (NLO polymers excited by surface plasmon enhanced optical fields. The surface plasmon (SP polariton was excited in an attenuated total reflection geometry having the Kretchmann configuration. The NLO polymers, consisting of Disperse Red1 as guest chromophores and poly (methyl methacrylate as host materials, were coated upon the Ag layers. Our experimental results indicated that the SHG signal intensity from the polymer coated Ag films was more than 10 times higher than that from the non-coated Ag films. The SHG autocorrelation traces excited by SP-enhanced fields were also studied and the correlation time was shorter than 150 fs, the temporal resolutions of the present spectrometer.

  3. Electron emission from insulator and semiconductor surfaces by multiphoton excitation below the optical damage threshold

    Science.gov (United States)

    Siekhaus, W. J.; Kinney, J. H.; Milam, D.; Chase, L. L.

    1986-03-01

    Electron emission due to 1.06 and 0.35 μm laser excitation has been measured at several pulse lengths for a number of wide bandgap semiconductors and insulators. The dependence on fluence and wavelength is consistent with multiphoton excitation across the bandgap. The work functions of the materials investigated do not appear to influence the rate-limiting multiphoton excitation process.

  4. Optical emission spectroscopy of excited atoms sputtered on a Ti surface under irradiation with multicharged Ar ions

    Energy Technology Data Exchange (ETDEWEB)

    Motohashi, K [Department of Applied Physics, Tokyo University of Agriculture and Technology, 2-24-16 Koganei-shi, Tokyo 184-8588 (Japan); Saitoh, Y [Department of Advanced Radiation Technology, Takasaki Advanced Radiation Research Institute, Japan Atomic Energy Agency (JAEA), Takasaki, Gunma 370-1292 (Japan); Kitazawa, S, E-mail: motohasi@cc.tuat.ac.j [Division of ITER Project, Fusion Research Development, Japan Atomic Energy Agency (JAEA), Naka, Ibaraki 311-0193 (Japan)

    2009-04-01

    Optical emission spectroscopy of excited atoms was carried out in order to investigate the sputtering processes on solid surfaces under irradiation of slow, multicharged ions. Many atomic lines of Ti I (neutral) and Ti II (single-charged ions) were observed in wavelengths from 250 to 750 nm with irradiation by Ar{sup 3+} (30 keV) on a Ti surface which was placed in a low pressure O{sub 2} atmosphere. The emission intensity of Ti I (520 nm) decreased monotonically with an increase of O{sub 2} partial pressure, whereas that of Ti I / II (670 nm, a 2nd order wavelength of 335 nm) slightly increased. From a semi-logarithmic plot of emission intensity for the 670 nm spectrum as a function of distance from the surface, the mean velocity of the excited Ti atoms and ions in a normal direction parallel to the surface, or

  5. Dissipative instability of a highly relativistic electron beam through the excitation of surface waves on a conducting medium

    Energy Technology Data Exchange (ETDEWEB)

    Shokri, B. [Physics Department and Laser-Plasma Research Institute of Shahid Beheshti University, Tehran (Iran, Islamic Republic of) and Institute for Studies in Theoretical Physics and Mathematics, P.O. Box 19395-1795, Tehran (Iran, Islamic Republic of)]. E-mail: b-shokri@cc.sbu.ac.ir; Khorashadizadeh, S.M. [Physics Department of Shahid Beheshti University, Tehran (Iran, Islamic Republic of); Physics Department of Birjand University, Birjand (Iran, Islamic Republic of)

    2005-09-19

    The possibility of the dissipative instability of a relativistic electron beam streaming near a conducting medium is investigated. The development of this dissipative beam instability through the surface wave excitation slightly disturbs the beam leading to the slightly heating of the conducting medium.

  6. Dynamical and scale invariance of charged particles slipping on a rough surface with periodic excitation

    Science.gov (United States)

    Zhang, Hao; Luo, Pengcheng; Ding, Huifang

    2017-07-01

    This letter deals with the dynamical and scaling invariance of charged particles slipping on a rough surface with periodic excitation. A variant of the Fermi-Ulam model (FUM) is proposed to describe the transport behavior of the particles when the electric field force Fe is smaller or larger than the friction force Ff, i.e., A 0. For these two cases, the stability of fixed points is analyzed with the help of the eigenvalue analysis method, and further the invariant manifolds are constructed to investigate the dynamical invariance such as energy diffusion for some initial conditions in the case A > 0 and decay process in the case A law of the statistical behavior. It follows that both the FA phenomenon for A > 0 and the velocity decay process for A < 0 satisfy scaling invariance with respect to the nondimensional acceleration A. Besides, for A < 0, the transient number nx is proposed to evaluate the speed of the velocity decay process. More importantly, nx is found to possess the attribute of scaling invariance with respect to both the initial velocity V0 and the nondimensional acceleration A. These results are very useful for the in-depth understanding of the energy transport properties of charged particle systems.

  7. Comprehensive analysis of photonic nanojets in 3D dielectric cuboids excited by surface plasmons

    Energy Technology Data Exchange (ETDEWEB)

    Pacheco-Pena, Victor [Antennas Group - TERALAB, Universidad Publica de Navarra, Campus Arrosadia, 31006, Pamplona (Spain); Minin, Igor V.; Minin, Oleg V. [National Research Tomsk State University, Lenina Ave., 36, Tomsk, 634050 (Russian Federation); Beruete, Miguel [Antennas Group - TERALAB, Universidad Publica de Navarra, Campus Arrosadia, 31006, Pamplona (Spain); Institute of Smart Cities, Public University of Navarra, 31006, Pamplona (Spain)

    2016-10-15

    In this paper we study the excitation of photonic nanojets (PNJ) in 3D dielectric cuboids by surface plasmons at telecommunication wavelengths. The analysis is done using the effective refractive index approach. It is shown that the refractive index contrast between the regions with and without cuboid should be roughly less than 2 in order to generate jets at the output of the cuboid. The best performance at λ{sub 0} = 1550 nm is obtained when the height of the cuboid is 160 nm producing a jet just at the output interface with a subwavelength resolution of 0.68λ{sub 0} and a high intensity enhancement (x 5) at the focus. The multi-wavelength response is also studied demonstrating that it is possible to use the proposed structure at different wavelengths. Finally, the backscattering enhancement is numerically evaluated by inserting a metal particle within the PNJ region, demonstrating a maximum value of ∝2.44 dB for a gold sphere of radius 0.1λ{sub 0}. (copyright 2016 by WILEY-VCH Verlag GmbH and Co. KGaA, Weinheim)

  8. Family of graphene-assisted resonant surface optical excitations for terahertz devices

    Science.gov (United States)

    Lin, I-Tan; Liu, Jia-Ming; Tsai, Hsin-Cheng; Wu, Kaung-Hsiung; Syu, Jheng-Yuan; Su, Ching-Yuan

    2016-01-01

    The majority of the proposed graphene-based THz devices consist of a metamaterial that can optically interact with graphene. This coupled graphene-metamaterial system gives rise to a family of resonant modes such as the surface plasmon polariton (SPP) modes of graphene, the geometrically induced SPPs, also known as the spoof SPP modes, and the Fabry-Perot (FP) modes. In the literature, these modes are usually considered separately as if each could only exist in one structure. By contrast, in this paper, we show that even in a simple metamaterial structure such as a one-dimensional (1D) metallic slit grating, these modes all exist and can potentially interact with each other. A graphene SPP-based THz device is also fabricated and measured. Despite the high scattering rate, the effective SPP resonances can still be observed and show a consistent trend between the effective frequency and the grating period, as predicted by the theory. We also find that the excitation of the graphene SPP mode is most efficient in the terahertz spectral region due to the Drude conductivity of graphene in this spectral region. PMID:27739504

  9. Magnification of photonic crystal fluorescence enhancement via TM resonance excitation and TE resonance extraction on a dielectric nanorod surface

    Energy Technology Data Exchange (ETDEWEB)

    Wu, Hsin-Yu; Cunningham, Brian T [Department of Electrical and Computer Engineering, University of Illinois at Urbana-Champaign, 1406 W Green Street, Urbana, IL 61801 (United States); Zhang Wei [Department of Material Science and Engineering, University of Illinois at Urbana-Champaign, 1304 W Green Street, Urbana, IL 61801 (United States); Mathias, Patrick C, E-mail: bcunning@illinois.edu [Department of Bioengineering, University of Illinois at Urbana-Champaign, 1304 W Springfield Avenue, Urbana, IL 61801 (United States)

    2010-03-26

    Using a one-dimensional grating surface photonic crystal (PC), we experimentally demonstrate that the detection of fluorescent molecules on a PC surface can be substantially magnified through the combined effects of resonance-enhanced excitation of the fluorescent dye, resonance-enhanced extraction of the fluorescence emission and a dielectric nanorod surface coating increasing the surface area available for fluorophore-PC interaction. Enhanced excitation is obtained by engineering a high-Q TM resonant mode to efficiently couple with an incident TM-polarized {lambda} = 633 nm laser for exciting Cyanine-5 (Cy5). Enhanced extraction results from a low-Q TE resonance designed to spectrally overlap the Cy5 emission spectrum for channeling TE-polarized emission towards the detection instrument. The entire PC surface is coated with a porous film of TiO{sub 2} nanorods that allows more fluorophores to penetrate into the region of enhanced near-electric fields. Experimental results reveal a 588-fold enhancement in fluorescence intensity relative to an unpatterned glass surface.

  10. ARTICLES: A Surface Femtosecond Two-Photon Photoemission Spectrometer for Excited Electron Dynamics and Time-Dependent Photochemical Kinetics

    Science.gov (United States)

    Ren, Ze-feng; Zhou, Chuan-yao; Ma, Zhi-bo; Xiao, Chun-lei; Mao, Xin-chun; Dai, Dong-xu; LaRue, Jerry; Cooper, Russell; Wodtke, Alec M.; Yang, Xue-ming

    2010-06-01

    A surface femtosecond two-photon photoemission (2PPE) spectrometer devoted to the study of ultrafast excited electron dynamics and photochemical kinetics on metal and metal oxide surfaces has been constructed. Low energy photoelectrons are measured using a hemispherical electron energy analyzer with an imaging detector that allows us to detect the energy and the angular distributions of the photoelectrons simultaneously. A Mach-Zehnder interferometer was built for the time-resolved 2PPE (TR-2PPE) measurement to study ultrafast surface excited electron dynamics, which was demonstrated on the Cu(111) surface. A scheme for measuring time-dependent 2PPE (TD-2PPE) spectra has also been developed for studies of surface photochemistry. This technique has been applied to a preliminary study on the photochemical kinetics on ethanol/TiO2(110). We have also shown that the ultrafast dynamics of photoinduced surface excited resonances can be investigated in a reliable way by combining the TR-2PPE and TD-2PPE techniques.

  11. Insight into the spin state at the surface of LaCoO3 revealed by photoemission electron microscopy

    Science.gov (United States)

    Yaroslavtsev, A. A.; Izquierdo, M.; Carley, R.; Dávila, M. E.; Ünal, A. A.; Kronast, F.; Lichtenstein, A.; Scherz, A.; Molodtsov, S. L.

    2016-04-01

    The evolution of the spin transition in LaCoO3 has been investigated with photoemission electron microscopy (PEEM) as a function of temperature. The investigated temperature range spanned from a predominantly low spin configuration (125 K) to the proposed percolation limit for metallization (413 K). The data show that the spin configuration exhibits an inhomogeneous spatial distribution that is very sensitive to the surface preparation method. In the region of the semiconductor-to-metal transition (300 to 450 K), the spatial contrast is continuously reduced, indicating a smooth transition without domain percolation. These observations support a new interpretation of the temperature evolution of the system that is in agreement with current theoretical understanding of the spin transition.

  12. Optical Diode Effect at Spin-Wave Excitations of the Room-Temperature Multiferroic BiFeO3

    Science.gov (United States)

    Kézsmárki, I.; Nagel, U.; Bordács, S.; Fishman, R. S.; Lee, J. H.; Yi, Hee Taek; Cheong, S.-W.; Rõõm, T.

    2015-09-01

    Multiferroics permit the magnetic control of the electric polarization and the electric control of the magnetization. These static magnetoelectric (ME) effects are of enormous interest: The ability to read and write a magnetic state current-free by an electric voltage would provide a huge technological advantage. Dynamic or optical ME effects are equally interesting, because they give rise to unidirectional light propagation as recently observed in low-temperature multiferroics. This phenomenon, if realized at room temperature, would allow the development of optical diodes which transmit unpolarized light in one, but not in the opposite, direction. Here, we report strong unidirectional transmission in the room-temperature multiferroic BiFeO3 over the gigahertz-terahertz frequency range. The supporting theory attributes the observed unidirectional transmission to the spin-current-driven dynamic ME effect. These findings are an important step toward the realization of optical diodes, supplemented by the ability to switch the transmission direction with a magnetic or electric field.

  13. Optical Diode Effect at Spin-Wave Excitations of the Room-Temperature Multiferroic BiFeO_{3}.

    Science.gov (United States)

    Kézsmárki, I; Nagel, U; Bordács, S; Fishman, R S; Lee, J H; Yi, Hee Taek; Cheong, S-W; Rõõm, T

    2015-09-18

    Multiferroics permit the magnetic control of the electric polarization and the electric control of the magnetization. These static magnetoelectric (ME) effects are of enormous interest: The ability to read and write a magnetic state current-free by an electric voltage would provide a huge technological advantage. Dynamic or optical ME effects are equally interesting, because they give rise to unidirectional light propagation as recently observed in low-temperature multiferroics. This phenomenon, if realized at room temperature, would allow the development of optical diodes which transmit unpolarized light in one, but not in the opposite, direction. Here, we report strong unidirectional transmission in the room-temperature multiferroic BiFeO_{3} over the gigahertz-terahertz frequency range. The supporting theory attributes the observed unidirectional transmission to the spin-current-driven dynamic ME effect. These findings are an important step toward the realization of optical diodes, supplemented by the ability to switch the transmission direction with a magnetic or electric field.

  14. Surface sensitivity of the spin Seebeck effect in the Pt/YIG system

    Science.gov (United States)

    Aqeel, Aisha; Vera-Marun, Ivan J.; van Wees, Bart J.; Palstra, Thomas T. M.

    2015-03-01

    It is well-known that the surface plays an important role in the spin Seebeck effect (SSE). However the effect of mechanical treatment on the SSE has not been systematically studied yet. Here, we have investigated the influence of the interface quality on the SSE in a bilayer system of platinum and yttrium iron garnet (Pt/YIG). The surfaces of the YIG crystals are modified by different types of mechanical polishing before Pt deposition for different samples. We observed that the magnitude and magnetic field dependence of the SSE is strongly influenced by mechanical treatment of the YIG surface. No definite relation has been found between the SSE response and the sample roughness. However, we observe a direct correlation between the saturation magnetic field (Hsat) of the SSE and the roughness of sample, as the former increases by moving from soft toward coarse particle polishing. The change in the magnitude of Hsat can be attributed to the presence of a perpendicular magnetic anisotropy due to the treatment induced surface strain or shape anisotropy in the Pt/YIG system.

  15. Spin-Casting Polymer Brush Films for Stimuli-Responsive and Anti-Fouling Surfaces.

    Science.gov (United States)

    Xu, Binbin; Feng, Chun; Hu, Jianhua; Shi, Ping; Gu, Guangxin; Wang, Lei; Huang, Xiaoyu

    2016-03-01

    Surfaces modified with amphiphilic polymers can dynamically alter their physicochemical properties in response to changes of their environmental conditions; meanwhile, amphiphilic polymer coatings with molecular hydrophilic and hydrophobic patches, which can mitigate biofouling effectively, are being actively explored as advanced coatings for antifouling materials. Herein, a series of well-defined amphiphilic asymmetric polymer brushes containing hetero side chains, hydrophobic polystyrene (PS) and hydrophilic poly(ethylene glycol) (PEG), was employed to prepare uniform thin films by spin-casting. The properties of these films were investigated by water contact angle, X-ray photoelectron spectroscopy (XPS), atomic force microscopy (AFM), and quartz crystal microbalance (QCM). AFM showed smooth surfaces for all films with the roughness less than 2 nm. The changes in water contact angle and C/O ratio (XPS) evidenced the enrichment of PEG or PS chains at film surface after exposed to selective solvents, indicative of stimuli- responsiveness. The adsorption of proteins on PEG functionalized surface was quantified by QCM and the results verified that amphiphilic polymer brush films bearing PEG chains could lower or eliminate protein-material interactions and resist to protein adsorption. Cell adhesion experiments were performed by using HaCaT cells and it was found that polymer brush films possess good antifouling ability.

  16. Elasto-dynamic analysis of spinning nanodisks via a surface energy-based model

    Science.gov (United States)

    Kiani, Keivan

    2016-07-01

    Using the surface elasticity theory of Gurtin and Murdoch, in-plane vibrations of annular nanodisks due to their rotary motion are explored. By the imposition of non-classical boundary conditions on the innermost and outermost surfaces and employing Hamilton’s principle, the unknown elasto-dynamic fields of the bulk zone are determined via the finite element method. The roles of both nanodisk geometry and surface effect on the natural frequencies are addressed. Subsequently, forced vibrations of spinning nanodisks with fixed-free and free-free boundary conditions are comprehensively examined. The obtained results show that the maximum dynamic elastic fields grow in a parabolic manner as the steady angular velocity increases. By increasing the outermost radius, the maximum dynamic elastic field is magnified and the influence of the surface effect on the results reduced. This work can be considered as a pivotal step towards optimal design and dynamic analysis of nanorotors with disk-like parts, which are one of the basic building blocks of the upcoming advanced nanotechnologies.

  17. Surface plasmon polariton excitation by electrostatic modulation and phase grating in indium-tin-oxide coated lithium niobate slabs

    Energy Technology Data Exchange (ETDEWEB)

    Wang, Hao; Zhang, Jingwen; Zhao, Hua, E-mail: zhaohuaz@hit.edu.cn [Institute of Modern Optics, Department of Physics, Harbin Institute of Technology, Harbin 150001 (China); Key Laboratory of Micro-Optics and Photonics Technology of Heilongjiang Province, Harbin 150001 (China)

    2015-08-14

    Excitation of surface plasmon polaritons (SPPs) in a non-metal system in visible regime is discussed. With the assistance of phase grating resulted from photorefractive effect and electrostatic modulation of ITO induced by strong photovoltaic effect in iron-doped LiNbO{sub 3}, phase matching condition could be satisfied for SPP excitation in this semiconductor/dielectric system. Both the phase grating instead of metal grating and electrostatic modulation of semiconductor could be used for the design of tunable plasmonic devices based on nonlinear photorefractive crystals.

  18. Surface Plasmon-Assisted Excitation of Atomic Visible Light Spectral Lines in the Impact of Highly Charged Ions 126Xeq+ on Solid Surfaces

    Institute of Scientific and Technical Information of China (English)

    张小安; 赵永涛; 李福利; 杨治虎; 肖国青; 詹文龙

    2003-01-01

    We measured the visible light spectral lines of sputtering atoms from solid surfaces of Al, Ti, Ni, Ta and Au which are impacted by 150keV126Xeq+ (6≤q≤30). It is found that intensities of the light spectral lines are greatly and suddenly enhanced when the charge state of the ion is raised up to a critical value. If assuming that potential energy released from the incidention due to capturing one electron is enough to excite a surface plasmon, we can estimate the critical charge states and obtain the results very well consistent with the measurements for the above-mentioned target materials. This means that a surface plasmon induced by one electron capture can enhance the excitation of atomic visible light spectral lines in the impact of a highly charged ion on a solid surface.

  19. Spin-polarized electronic structure of the Ni(001) surface and thin films

    DEFF Research Database (Denmark)

    Jepsen, O.; Madsen, J.; Andersen, O. K.

    1982-01-01

    of the five-layer film is used to calculate the electronic structure of a 13-layer film. The theoretical work function of 5.4 eV agrees well with the experimental value of 5.2 eV. The calculated spin moments are ordered ferromagnetically in all the films considered, and the moments of the atoms in the surface...... layer are 0.95, 0.69, and 0.65 Bohr magnetons for the one-, three-, and five-layer films, respectively. The moment of an atom in the central layer of the five-layer film is 0.61 Bohr magnetons as compared with the calculated (experimental) bulk value of 0.59±0.01 (0.56) Bohr magnetons. The increase...

  20. Observation of second spin reorientation transition within ultrathin region in Fe films on Ag(001) surface

    Energy Technology Data Exchange (ETDEWEB)

    Khim, T.-Y. [c-CCMR and Department of Physics, POSTECH, Pohang 790-784 (Korea, Republic of); Shin, M.; Lee, H., E-mail: easyscan@sookmyung.ac.kr, E-mail: jhp@postech.ac.kr [Department of Chemistry, Sookmyung Women' s University, Seoul 140-742 (Korea, Republic of); Park, B.-G. [Pohang Accelerator Laboratory (PAL), Pohang 790-784 (Korea, Republic of); Park, J.-H., E-mail: easyscan@sookmyung.ac.kr, E-mail: jhp@postech.ac.kr [c-CCMR and Department of Physics, POSTECH, Pohang 790-784 (Korea, Republic of); Division of Advanced Materials Science, POSTECH, Pohang 790-784 (Korea, Republic of); Max Plank POSTECH Center for Complex Phase Materials, POSTECH, Pohang 790-784 (Korea, Republic of)

    2014-06-21

    We acquired direct measurements for in-plane and perpendicular-to-plane magnetic moments of Fe films using an x-ray magnetic circular dichroism technique with increase of the Fe thickness (up to 40 Å) on the Ag(001) surface. Epitaxial Fe/Ag(001) films were grown in situ with the thickness varying from 2 Å to 40 Å, and the magnetic anisotropy was carefully investigated as a function of the film thickness. We found re-entrance of the in-plane magnetic anisotropy of the Fe film in ultrathin region. The results manifest that the epitaxial Fe/Ag(001) film undergoes two distinct spin reorientation transitions from in-plane to out-of-plane at the film thickness t ≈ 9 Å and back to in-plane at t ≈ 18 Å as t increases.

  1. Characterization of silanization and antibody immobilization on spin-on glass (SOG) surface

    Energy Technology Data Exchange (ETDEWEB)

    Nagare, Gajanan D. [School of Biosciences and Bio-Engineering, IIT Bombay (India); Mukherji, S. [School of Biosciences and Bio-Engineering, IIT Bombay (India)], E-mail: mukherji@iitb.ac.in

    2009-01-01

    Most embedded optical waveguide biosensors require low dielectric optical material. The prerequisites for such applications include the selection of an appropriate material and effective bio-functionalization. Spin-on glass (SOG) is one of the preferred polymers that can be easily deposited. Further, the chemical properties of the polymer make it amenable for bio-functionalization. This paper reports a detailed study of a protocol for immobilization of antibodies on SOG for possible immunobiosensor applications. The effect of silanization at different pH values on the number of free and usable amine sites was quantified by fluorimetry. Contact angle measurements, ellipsometry, AFM, and fluorescence microscopy was used for assessing the surface properties at various stages of preparation, functionalization and biomolecule immobilization.

  2. Giant spin splitting of the two-dimensional electron gas at the surface of SrTiO3

    Science.gov (United States)

    Santander-Syro, A. F.; Fortuna, F.; Bareille, C.; Rödel, T. C.; Landolt, G.; Plumb, N. C.; Dil, J. H.; Radović, M.

    2014-12-01

    Two-dimensional electron gases (2DEGs) forming at the interfaces of transition metal oxides exhibit a range of properties, including tunable insulator-superconductor-metal transitions, large magnetoresistance, coexisting ferromagnetism and superconductivity, and a spin splitting of a few meV (refs , ). Strontium titanate (SrTiO3), the cornerstone of such oxide-based electronics, is a transparent, non-magnetic, wide-bandgap insulator in the bulk, and has recently been found to host a surface 2DEG (refs , , , ). The most strongly confined carriers within this 2DEG comprise two subbands, separated by an energy gap of 90 meV and forming concentric circular Fermi surfaces. Using spin- and angle-resolved photoemission spectroscopy (SARPES), we show that the electron spins in these subbands have opposite chiralities. Although the Rashba effect might be expected to give rise to such spin textures, the giant splitting of almost 100 meV at the Fermi level is far larger than anticipated. Moreover, in contrast to a simple Rashba system, the spin-polarized subbands are non-degenerate at the Brillouin zone centre. This degeneracy can be lifted by time-reversal symmetry breaking, implying the possible existence of magnetic order. These results show that confined electronic states at oxide surfaces can be endowed with novel, non-trivial properties that are both theoretically challenging to anticipate and promising for technological applications.

  3. Conservation laws, radiative decay rates, and excited state localization in organometallic complexes with strong spin-orbit coupling

    CERN Document Server

    Powell, B J

    2015-01-01

    There is longstanding fundamental interest in 6-fold coordinated $d^6$ ($t_{2g}^6$) transition metal complexes such as [Ru(bpy)$_3$]$^{2+}$ and Ir(ppy)$_3$, particularly their phosphorescence. This interest has increased with the growing realisation that many of these complexes have potential uses in applications including photovoltaics, imaging, sensing, and light-emitting diodes. In order to design new complexes with properties tailored for specific applications a detailed understanding of the low-energy excited states, particularly the lowest energy triplet state, $T_1$, is required. Here we describe a model of pseudo-octahedral complexes based on a pseudo-angular momentum representation and show that the predictions of this model are in excellent agreement with experiment - even when the deviations from octahedral symmetry are large. This model gives a natural explanation of zero-field splitting of $T_1$ and of the relative radiative rates of the three sublevels in terms of the conservation of time-revers...

  4. Dynamics of sessile and pendant drop excited by surface acoustic waves: gravity effects and correlation between oscillatory and translational motions

    CERN Document Server

    Bussonière, Adrien; Brunet, Philippe; Matar, Olivier Bou

    2016-01-01

    When sessile droplets are excited by ultrasonic traveling surface acoustic waves (SAWs), they undergo complex dynamics with both oscillations and translational motion. While the nature of the Rayleigh-Lamb quadrupolar drop oscillations has been identified, their origin and their influence on the drop mobility remains unexplained. Indeed the physics behind this peculiar dynamics is complex with nonlinearities involved both at the excitation level (acoustic streaming and radiation pressure) and in the droplet response (nonlinear oscillations and contact line dynamics). In this paper, we investigate the dynamics of sessile and pendant drops excited by SAWs. For pendant drops, so-far unreported dynamics are observed close to the drop detachment threshold with the suppression of the translational motion. Away from this threshold, the comparison between pendant and sessile drop dynamics allows us to identify the role played by gravity or more generally by an initial or dynamically induced stretching of the drop. In...

  5. Excitation of the Slichter mode by collision with a meteoroid or pressure variations at the surface and core boundaries

    CERN Document Server

    Rosat, S; 10.1016/J.PEPI.2011.10.007

    2012-01-01

    We use a normal-mode formalism to compute the response of a spherical, self-gravitating anelastic PREM-like Earth model to various excitation sources at the Slichter mode period. The formalism makes use of the theory of the Earth's free oscillations based upon an eigenfunction expansion methodology. We determine the complete response in the form of Green's function obtained from a generalization of Betti's reciprocity theorem. Surficial (surface load, fluid core pressure), internal (earthquakes, explosions) and external (object impact) sources of excitation are investigated to show that the translational motion of the inner-core would be best excited by a pressure acting at the core boundaries at time-scales shorter than the Slichter eigenperiods.

  6. Versatile and tunable surface plasmon polariton excitation over a broad bandwidth with a simple metaline by external polarization modulation.

    Science.gov (United States)

    You, Oubo; Bai, Benfeng; Sun, Lin; Shen, Biyao; Zhu, Zhendong

    2016-09-19

    Surface plasmon polariton (SPP) sources and launchers are highly demanded in various applications of nanophotonics. Here, we propose a general approach that can realize complete control of the complex extinction ratio (including amplitude and phase) of any two linearly independent SPP modes excited by any elementary SPP excitation architecture just by manipulating the incident polarization state. In an optical system, it suffices to simply tune the orientation angles of a linear polarizer and a quarter wave plate, which may greatly simplify the design and application of SPP launchers and diversify their functionalities. As an example to show the broad application prospect of this method, we design and realize a metaline consisting of Δ-shaped plasmonic nanoantennas, which can effectively realize dual functionalities, i.e., the tunable directional SPP excitation at an arbitrarily chosen wavelength and the complete unidirectional SPP excitation over a broad bandwidth. This general approach can also be extended to the control of the complex extinction ratio of any two linearly independent excited modes in many other linear optical systems, such as two modes in a waveguide or two diffraction orders in a grating, over a broad bandwidth.

  7. Half-filled Landau level, topological insulator surfaces, and three-dimensional quantum spin liquids

    Science.gov (United States)

    Wang, Chong; Senthil, T.

    2016-02-01

    We synthesize and partly review recent developments relating the physics of the half-filled Landau level in two dimensions to correlated surface states of topological insulators in three dimensions. The latter are in turn related to the physics of certain three-dimensional quantum spin liquid states. The resulting insights provide an interesting answer to the old question of how particle-hole symmetry is realized in composite fermion liquids. Specifically the metallic state at filling ν =1/2 —described originally in pioneering work by Halperin, Lee, and Read as a liquid of composite fermions—was proposed recently by Son to be described by a particle-hole symmetric effective field theory distinct from that in the prior literature. We show how the relation to topological insulator surface states leads to a physical understanding of the correctness of this proposal. We develop a simple picture of the particle-hole symmetric composite fermion through a modification of older pictures as electrically neutral "dipolar" particles. We revisit the phenomenology of composite fermi liquids (with or without particle-hole symmetry), and show that their heat/electrical transport dramatically violates the conventional Wiedemann-Franz law but satisfies a modified one. We also discuss the implications of these insights for finding physical realizations of correlated topological insulator surfaces.

  8. Potential energy surface of excited semiconductors: Graphene quantum dot and BODIPY

    Science.gov (United States)

    Colherinhas, Guilherme; Fileti, Eudes Eterno; Chaban, Vitaly V.

    2016-08-01

    Binding energy (BE) is an important descriptor in chemistry, which determines thermodynamics and phase behavior of a given substance. BE between two molecules is not directly accessible from the experiment. It has to be reconstructed from cohesive energies, vaporization heats, etc. We report BE for the excited states of two semiconductor molecules - boron-dipyrromethene (BODIPY) and graphene quantum dot (GQD) - with water. We show, for the first time, that excitation increases BE twofold at an optimal separation (energy minimum position), whereas higher separations lead to higher differences. Interestingly, the effects of excitation are similar irrespective of the dominant binding interactions (van der Waals or electrostatic) in the complex. This new knowledge is important for simulations of the excited semiconductors by simplified interaction functions.

  9. Spin pumping and spin-orbit effects in Ge (Conference Presentation)

    Science.gov (United States)

    Oyarzún, Simón; Nandy, Ashis Kumar; Rortais, Fabien; Rojas-Sánchez, Juan Carlos; Laczkowski, Piotr; Pouget, Stephanie; Okuno, Hanako; Vila, Laurent; Vergnaud, Céline; Beigne, Cyrille; Marty, Alain; Attané, Jean Philippe; Gambarelli, Serge; George, Jean Marie; Jaffres, Henri; Blügel, Stefan; Jamet, Matthieu

    2016-10-01

    The field of spintronics is based on the manipulation of the spin degree of freedom. It uses the carrier spin angular momentum as a basic functional unit in addition to the charge. The first requirement of a semiconductor-based spintronic technology is the efficient generation of spin-polarized carriers into the device heterostructure made of Si or Ge (the materials of mainstream microelectronics) at room temperature. In this presentation, we focus on the generation of a sizeable spin population into Ge by spin pumping. Spin pumping corresponds to the generation of a pure spin current in the Ge film by exciting the ferromagnetic resonance of an adjacent ferromagnetic electrode with microwaves. The pure spin current is then detected using spin-orbit based effects. Our aim is to understand the basic mechanisms of spin pumping into Ge as well as the spin-to-charge conversion by inverse spin Hall effect (ISHE, bulk effect) [1-4] and Rashba-Edelstein effect (interface effect) [5]. The influence of interface states is clearly demonstrated. Moreover, using the spin-split Rashba sub-surface states of the Ge(111) surface, we succeeded in demonstrating a giant conversion of a spin current generated by spin pumping into a charge current by the Rashba-Edelstein effect [6,7]. Our experimental findings are supported by ab-initio calculations. 1. Rojas-Sánchez, J.-C. et al. Spin pumping and inverse spin Hall effect in germanium. Phys. Rev. B 88, (2013). 2. Kato, Y. K., Myers, R. C., Gossard, A. C. and Awschalom, D. D. Observation of the spin Hall effect in semiconductors. Science 306, 1910-1913 (2004). 3. Valenzuela, S. O. and Tinkham, M. Direct electronic measurement of the spin Hall effect. Nature 442, 176-179 (2006). 4. Saitoh, E., Ueda, M., Miyajima, H. and Tatara, G. Conversion of spin current into charge current at room temperature: Inverse spin-Hall effect. Appl Phys Lett 88, 2509 (2006). 5. Bychkov, Y. A. and Rashba, E. I. Oscillatory effects and the magnetic

  10. A highly efficient surface plasmon polaritons excitation achieved with a metal-coupled metal-insulator-metal waveguide

    Directory of Open Access Journals (Sweden)

    Hongyan Yang

    2014-12-01

    Full Text Available We propose a novel metal-coupled metal-insulator-metal (MC-MIM waveguide which can achieve a highly efficient surface plasmon polaritons (SPPs excitation. The MC-MIM waveguide is formed by inserting a thin metal film in the insulator of an MIM. The introduction of the metal film, functioning as an SPPs coupler, provides a space for the interaction between SPPs and a confined electromagnetic field of the intermediate metal surface, which makes energy change and phase transfer in the metal-dielectric interface, due to the joint action of incomplete electrostatic shielding effect and SPPs coupling. Impacts of the metal film with different materials and various thickness on SPPs excitation are investigated. It is shown that the highest efficient SPPs excitation is obtained when the gold film thickness is 60 nm. The effect of refractive index of upper and lower symmetric dielectric layer on SPPs excitation is also discussed. The result shows that the decay value of refractive index is 0.3. Our results indicate that this proposed MC-MIM waveguide may offer great potential in designing a new SPPs source.

  11. Characteristics of localized surface plasmons excited on mixed monolayers composed of self-assembled Ag and Au nanoparticles.

    Science.gov (United States)

    Tanaka, Daisuke; Imazu, Keisuke; Sung, Jinwoo; Park, Cheolmin; Okamoto, Koichi; Tamada, Kaoru

    2015-10-07

    The fundamental characteristics of localized surface plasmon resonance (LSPR) excited on mixed monolayers composed of self-assembled Ag and Au nanoparticles (AgNPs and AuNPs, respectively) were investigated. Mixed monolayered films were fabricated at the air-water interface at different mixing ratios. The films retained their phase-segregated morphologies in which AuNPs formed several 10 to 100 nm island domains in a homogeneous AgNP matrix phase. The LSPR bands originating from the self-assembled domains shifted to longer wavelengths as the domain size increased, as predicted by a finite-difference time-domain (FDTD) simulation. The FDTD simulation also revealed that even an alternating-lattice-structured two-dimensional (2D) AgNP/AuNP film retained two isolated LSPR bands, revealing that the plasmon resonances excited on each particle did not couple even in a continuous 2D sheet, unlike in the homologous NP system. The fluorescence quenching test of Cy3 and Cy5 dyes confirmed that the independent functions of AuNPs and AgNPs remained in the mixed films, whereas the AuNPs exhibited significantly higher quenching efficiency for the Cy3 dye compared with AgNPs due to the overlap of the excitation/emission bands of the dyes with the AuNP LSPR band. Various applications can be considered using this nanoheterostructured plasmonic assembly to excite spatially designed, high-density LSPR on macroscopic surfaces.

  12. Valence excitation energies of alkenes, carbonyl compounds, and azabenzenes by time-dependent density functional theory: Linear response of the ground state compared to collinear and noncollinear spin-flip TDDFT with the Tamm-Dancoff approximation

    Science.gov (United States)

    Isegawa, Miho; Truhlar, Donald G.

    2013-04-01

    Time-dependent density functional theory (TDDFT) holds great promise for studying photochemistry because of its affordable cost for large systems and for repeated calculations as required for direct dynamics. The chief obstacle is uncertain accuracy. There have been many validation studies, but there are also many formulations, and there have been few studies where several formulations were applied systematically to the same problems. Another issue, when TDDFT is applied with only a single exchange-correlation functional, is that errors in the functional may mask successes or failures of the formulation. Here, to try to sort out some of the issues, we apply eight formulations of adiabatic TDDFT to the first valence excitations of ten molecules with 18 density functionals of diverse types. The formulations examined are linear response from the ground state (LR-TDDFT), linear response from the ground state with the Tamm-Dancoff approximation (TDDFT-TDA), the original collinear spin-flip approximation with the Tamm-Dancoff (TD) approximation (SF1-TDDFT-TDA), the original noncollinear spin-flip approximation with the TDA approximation (SF1-NC-TDDFT-TDA), combined self-consistent-field (SCF) and collinear spin-flip calculations in the original spin-projected form (SF2-TDDFT-TDA) or non-spin-projected (NSF2-TDDFT-TDA), and combined SCF and noncollinear spin-flip calculations (SF2-NC-TDDFT-TDA and NSF2-NC-TDDFT-TDA). Comparing LR-TDDFT to TDDFT-TDA, we observed that the excitation energy is raised by the TDA; this brings the excitation energies underestimated by full linear response closer to experiment, but sometimes it makes the results worse. For ethylene and butadiene, the excitation energies are underestimated by LR-TDDFT, and the error becomes smaller making the TDA. Neither SF1-TDDFT-TDA nor SF2-TDDFT-TDA provides a lower mean unsigned error than LR-TDDFT or TDDFT-TDA. The comparison between collinear and noncollinear kernels shows that the noncollinear kernel

  13. Description of excited states in [Re(Imidazole)(CO)3 (Phen)](+) including solvent and spin-orbit coupling effects: Density functional theory versus multiconfigurational wavefunction approach.

    Science.gov (United States)

    Fumanal, Maria; Daniel, Chantal

    2016-10-15

    The low-lying electronic excited states of [Re(imidazole)(CO)3 (phen)](+) (phen = 1,10-phenanthroline) ranging between 420 nm and 330 nm have been calculated by means of relativistic spin-orbit time-dependent density functional theory (TD-DFT) and wavefunction approaches (state-average-CASSCF/CASPT2). A direct comparison between the theoretical absorption spectra obtained with different methods including SOC and solvent corrections for water points to the difficulties at describing on the same footing the bands generated by metal-to-ligand charge transfer (MLCT), intraligand (IL) transition, and ligand-to-Ligand- charge transfer (LLCT). While TD-DFT and three-roots-state-average CASSCF (10,10) reproduce rather well the lowest broad MLCT band observed in the experimental spectrum between 420 nm and 330 nm, more flexible wavefunctions enlarged either by the number of roots or by the number of active orbitals and electrons destabilize the MLCT states by introducing IL and LLCT character in the lowest part of the absorption spectrum. © 2016 Wiley Periodicals, Inc.

  14. Atomistic simulation of charge effects: From tunable thin film growth to isolation of surface states with spin-orbit coupling

    Science.gov (United States)

    Ming, Wenmei

    This dissertation revitalizes the importance of surface charge effects in semiconductor nanostructures, in particular in the context of thin film growth and exotic electronic structures under delicate spin-orbit coupling. A combination of simulation techniques, including density functional theory calculation, kinetic Monte Carlo method, nonequilibrium Green's function method, and tight binding method, were employed to reveal the underlying physical mechanisms of four topics: (1) Effects of Li doping on H-diffusion in MgH 2 for hydrogen storage. It addresses both the effect of Fermi level tuning by charged dopant and the effect of dopant-defect interaction, and the latter was largely neglected in previous works; (2) Tuning nucleation density of the metal island with charge doping of the graphene substrate. It is the first time that the surface charge doping effect is proposed and studied as an effective approach to tune the kinetics of island nucleation at the early stage of thin film growth; (3) Complete isolation of Rashba surface states on the saturated semiconductor surface. It shows that the naturally saturated semiconductor surface of InSe(0001) with Au single layer film provides a mechanism for the formation of Rashba states with large spin splitting; it opens up an innovative route to obtaining ideal Rashba states without the overwhelming bulk spin-degenerate carriers in spin-dependent transport; (4) Formation of large band gap quantum spin Hall state on Si surface. This study reveals the importance of atomic orbital composition in the formation of a topological insulator, and shows promisingly the possible integration of topological insulator technology into Si-based modern electronic devices.

  15. Spin-controlled plasmonics via optical Rashba effect

    Energy Technology Data Exchange (ETDEWEB)

    Shitrit, Nir; Yulevich, Igor; Kleiner, Vladimir; Hasman, Erez, E-mail: mehasman@technion.ac.il [Micro and Nanooptics Laboratory, Faculty of Mechanical Engineering, and Russell Berrie Nanotechnology Institute, Technion—Israel Institute of Technology, Haifa 32000 (Israel)

    2013-11-18

    Observation of the optical Rashba effect in plasmonics is reported. Polarization helicity degeneracy removal, associated with the inversion symmetry violation, is attributed to the surface symmetry design via anisotropic nanoantennas with space-variant orientations. By utilizing the Rashba-induced momentum in a nanoscale kagome metastructure, we demonstrated a spin-based surface plasmon multidirectional excitation under a normal-incidence illumination. The spin-controlled plasmonics via spinoptical metasurfaces provides a route for spin-based surface-integrated photonic nanodevices and light-matter interaction control, extending the light manipulation capabilities.

  16. Ab initio ground and excited state potential energy surfaces for NO-Kr complex and dynamics of Kr solids with NO impurity.

    Science.gov (United States)

    Castro-Palacios, Juan Carlos; Rubayo-Soneira, Jesús; Ishii, Keisaku; Yamashita, Koichi

    2007-04-01

    The intermolecular potentials for the NO(X 2Pi)-Kr and NO(A 2Sigma+)-Kr systems have been calculated using highly accurate ab initio calculations. The spin-restricted coupled cluster method for the ground 1 2A' state [NO(X 2Pi)-Kr] and the multireference singles and doubles configuration interaction method for the excited 2 2A' state [NO(A 2Sigma+)-Kr], respectively, were used. The potential energy surfaces (PESs) show two linear wells and one that is almost in the perpendicular position. An analytical representation of the PESs has been constructed for the triatomic systems and used to carry out molecular dynamics (MD) simulations of the NO-doped krypton matrix response after excitation of NO. MD results are shown comparatively for three sets of potentials: (1) anisotropic ab initio potentials [NO molecule direction fixed during the dynamics and considered as a point (its center of mass)], (2) isotropic ab initio potentials (isotropic part in a Legendre polynomial expansion of the PESs), and (3) fitted Kr-NO potentials to the spectroscopic data. An important finding of this work is that the anisotropic and isotropic ab initio potentials calculated for the Kr-NO triatomic system are not suitable for describing the dynamics of structural relaxation upon Rydberg excitation of a NO impurity in the crystal. However, the isotropic ab initio potential in the ground state almost overlaps the published experimental potential, being almost independent of the angle asymmetry. This fact is also manifested in the radial distribution function around NO. However, in the case of the excited state the isotropic ab initio potential differs from the fitted potentials, which indicates that the Kr-NO interaction in the matrix is quite different because of the presence of the surrounding Kr atoms acting on the NO molecule. MD simulations for isotropic potentials reasonably reproduce the experimental observables for the femtosecond response and the bubble size but do not match

  17. Linear in-plane magnetoconductance and spin susceptibility of a 2D electron gas on a vicinal silicon surface

    OpenAIRE

    Proskuryakov, Y. Y.; Kvon, Z. D.; Savchenko, A. K.

    2003-01-01

    In this work we have studied the parallel magnetoresistance of a 2DEG near a vicinal silicon surface. An unusual, linear magnetoconductance is observed in the fields up to $B = 15$ T, which we explain by the effect of spin olarization on impurity scattering. This linear magnetoresistance shows strong anomalies near the boundaries of the minigap in the electron spectrum of the vicinal system.

  18. Magnetization switching of a metallic nanomagnet via current-induced surface spin-polarization of an underlying topological insulator

    Energy Technology Data Exchange (ETDEWEB)

    Roy, Urmimala; Dey, Rik; Pramanik, Tanmoy; Ghosh, Bahniman; Register, Leonard F.; Banerjee, Sanjay K. [Microelectronics Research Center, The University of Texas at Austin, Austin, Texas 78758 (United States)

    2015-04-28

    We consider a thermally stable, metallic nanoscale ferromagnet (FM) subject to spin-polarized current injection and exchange coupling from the spin-helically locked surface states of a topological insulator (TI) to evaluate possible non-volatile memory applications. We consider parallel transport in the TI and the metallic FM, and focus on the efficiency of magnetization switching as a function of transport between the TI and the FM. Transport is modeled as diffusive in the TI beneath the FM, consistent with the mobility in the TI at room temperature, and in the FM, which essentially serves as a constant potential region albeit spin-dependent except in the low conductivity, diffusive limit. Thus, it can be captured by drift-diffusion simulation, which allows for ready interpretation of the results. We calculate switching time and energy consumed per write operation using self-consistent transport, spin-transfer-torque (STT), and magnetization dynamics calculations. Calculated switching energies and times compare favorably to conventional spin-torque memory schemes for substantial interlayer conductivity. Nevertheless, we find that shunting of current from the TI to a metallic nanomagnet can substantially limit efficiency. Exacerbating the problem, STT from the TI effectively increases the TI resistivity. We show that for optimum performance, the sheet resistivity of the FM layer should be comparable to or larger than that of the TI surface layer. Thus, the effective conductivity of the FM layer becomes a critical design consideration for TI-based non-volatile memory.

  19. Magnetization switching of a metallic nanomagnet via current-induced surface spin-polarization of an underlying topological insulator

    Science.gov (United States)

    Roy, Urmimala; Dey, Rik; Pramanik, Tanmoy; Ghosh, Bahniman; Register, Leonard F.; Banerjee, Sanjay K.

    2015-04-01

    We consider a thermally stable, metallic nanoscale ferromagnet (FM) subject to spin-polarized current injection and exchange coupling from the spin-helically locked surface states of a topological insulator (TI) to evaluate possible non-volatile memory applications. We consider parallel transport in the TI and the metallic FM, and focus on the efficiency of magnetization switching as a function of transport between the TI and the FM. Transport is modeled as diffusive in the TI beneath the FM, consistent with the mobility in the TI at room temperature, and in the FM, which essentially serves as a constant potential region albeit spin-dependent except in the low conductivity, diffusive limit. Thus, it can be captured by drift-diffusion simulation, which allows for ready interpretation of the results. We calculate switching time and energy consumed per write operation using self-consistent transport, spin-transfer-torque (STT), and magnetization dynamics calculations. Calculated switching energies and times compare favorably to conventional spin-torque memory schemes for substantial interlayer conductivity. Nevertheless, we find that shunting of current from the TI to a metallic nanomagnet can substantially limit efficiency. Exacerbating the problem, STT from the TI effectively increases the TI resistivity. We show that for optimum performance, the sheet resistivity of the FM layer should be comparable to or larger than that of the TI surface layer. Thus, the effective conductivity of the FM layer becomes a critical design consideration for TI-based non-volatile memory.

  20. High-sensitivity label-free optical fiber optrodes based on the excitation of Bloch surface waves

    Science.gov (United States)

    Scaravilli, M.; Castaldi, G.; Cusano, A.; Galdi, V.

    2016-05-01

    In this study, the possibility to excite Bloch surface waves (BSWs) on the tip of a single-mode optical fiber is explored for the first time. In particular, we first show the possibility to achieve an on-tip excitation of BSWs, with optimized characteristic of the arising resonances, via an "all-fiber" grating-coupled configuration. Furthermore, envisioning novel high-performance fiber tip nanoprobes for label-free biosensing, we introduce an ad hoc design aimed at maximizing the refractive-index sensitivity. Numerical results indicate that the estimated sensitivities are comparable with those exhibited by current plasmonic lab-on-tip bio-probes, but are accompanied by a higher spectral selectivity. Therefore, this preliminary work paves the way to the development of new classes of miniaturized surface-wave optical fiber devices for low-detection-limit label-free chemical and biological sensing.

  1. Diagnostics of the efficiency of surface plasmon-polariton excitation by quantum dots via polarization measurements of the output radiation

    Energy Technology Data Exchange (ETDEWEB)

    Kukushkin, V. A., E-mail: vakuk@appl.sci-nnov.ru [Russian Academy of Sciences, Institute of Applied Physics (Russian Federation); Baidus, N. V. [Lobachevsky State University of Nizhni Novgorod (Russian Federation); Zdoroveishchev, A. V. [Lobachevsky State University of Nizhni Novgorod, Physicotechnical Research Institute (Russian Federation)

    2015-06-15

    It is demonstrated that the efficiency of surface plasmon-polariton excitation at a metal-semiconductor interface by active quantum dots can be determined from measurements of the polarization characteristics of the output radiation. Experimentally, the proposed diagnostic method is based on finding the ratio of the intensities of the output radiation with polarizations orthogonal and parallel to the nanoheterostructure plane for two different distances between the quantum-dot layer and the metal-semiconductor interface. These data are then used to obtain the unknown parameters in the proposed mathematical model which makes it possible to calculate the rate of surface plasmon-polariton excitation by active quantum dots. As a result, this rate can be determined without complicated expensive equipment for fast time-resolved measurements.

  2. Spin-orbit coupled potential energy surfaces and properties using effective relativistic coupling by asymptotic representation

    Science.gov (United States)

    Ndome, Hameth; Eisfeld, Wolfgang

    2012-08-01

    A new method has been reported recently [H. Ndome, R. Welsch, and W. Eisfeld, J. Chem. Phys. 136, 034103 (2012)], 10.1063/1.3675846 that allows the efficient generation of fully coupled potential energy surfaces (PESs) including derivative and spin-orbit (SO) coupling. The method is based on the diabatic asymptotic representation of the molecular fine structure states and an effective relativistic coupling operator and therefore is called effective relativistic coupling by asymptotic representation (ERCAR). The resulting diabatic spin-orbit coupling matrix is constant and the geometry dependence of the coupling between the eigenstates is accounted for by the diabatization. This approach allows to generate an analytical model for the fully coupled PESs without performing any ab initio SO calculations (except perhaps for the atoms) and thus is very efficient. In the present work, we study the performance of this new method for the example of hydrogen iodide as a well-established test case. Details of the diabatization and the accuracy of the results are investigated in comparison to reference ab initio calculations. The energies of the adiabatic fine structure states are reproduced in excellent agreement with reference ab initio data. It is shown that the accuracy of the ERCAR approach mainly depends on the quality of the underlying ab initio data. This is also the case for dissociation and vibrational level energies, which are influenced by the SO coupling. A method is presented how one-electron operators and the corresponding properties can be evaluated in the framework of the ERCAR approach. This allows the computation of dipole and transition moments of the fine structure states in good agreement with ab initio data. The new method is shown to be very promising for the construction of fully coupled PESs for more complex polyatomic systems to be used in quantum dynamics studies.

  3. Theory of optical excitation and relaxation phenomena at semiconductor surfaces: linking density functional and density matrix theory

    Energy Technology Data Exchange (ETDEWEB)

    Buecking, N. [Technische Universitaet Berlin, Institut fuer Theoretische Physik, Nichtlineare Optik und Quantenelektronik, Berlin (Germany); Fritz-Haber-Institut der Max-Planck-Gesellschaft, Berlin (Germany); Scheffler, M. [Fritz-Haber-Institut der Max-Planck-Gesellschaft, Berlin (Germany); Kratzer, P. [Universitaet Duisburg-Essen, Fachbereich Physik - Theoretische Physik, Duisburg (Germany); Knorr, A. [Technische Universitaet Berlin, Institut fuer Theoretische Physik, Nichtlineare Optik und Quantenelektronik, Berlin (Germany)

    2007-08-15

    A theory for the description of optical excitation and the subsequent phonon-induced relaxation dynamics of nonequilibrium electrons at semiconductor surfaces is presented. In the first part, the fundamental dynamical equations for electronic occupations and polarisations are derived using density matrix formalism (DMT) for a surface-bulk system including the interaction of electrons with the optical field and electron-phonon interactions. The matrix elements entering these equations are either determined empirically or by density functional theory (DFT) calculations. In the subsequent parts of the paper, the dynamics at two specific semiconductor surfaces are discussed in detail. The electron relaxation dynamics underlying a time-resolved two photon photoemission experiment at an InP surface is investigated in the limit of a parabolic four band model. Moreover, the electron relaxation dynamics at a Si(100) surface is analysed. Here, the coupling parameters and the band structure are obtained from an DFT calculations. (orig.)

  4. Spin pumping with coherent elastic waves

    Science.gov (United States)

    Weiler, M.; Huebl, H.; Goerg, F. S.; Czeschka, F. D.; Gross, R.; Goennenwein, S. T. B.

    2012-02-01

    The generation and detection of pure spin currents is an important topic for spintronic applications. Spin currents may be generated, e.g., via spin pumping. In this approach, a precessing magnetization relaxes via the emission of a spin current. Conventionally, electromagnetic waves, i.e. microwave photons, are used to drive the magnetization precession. We here show that a spin current can also be pumped by means of an acoustic wave, i.e. microwave phonons. In the experiments, coherent surface acoustic wave (SAW) phonons with a frequency of 1.55 GHz traverse a ferromagnetic thin film/normal metal (Co/Pt) bilayer. The SAW phonons drive the resonant magnetization precession via magnetoelastic coupling [1]. We use the inverse spin Hall voltage in the Pt film as a measure for the generated spin current and record its evolution as a function of time and external magnetic field magnitude and orientation. Our experiments show that a spin current is generated in the exclusive presence of a resonant elastic excitation. This establishes acoustic spin pumping as a resonant analogue to the spin Seebeck effect and opens intriguing perspectives for applications in, e.g., micromechanical resonators. [4pt] [1] M. Weiler et al., Phys. Rev. Lett. 106, 117601 (2011)

  5. Propagation of pulsed surface spin-wave signals at millikelvin temperatures

    Science.gov (United States)

    van Loo, Arjan; Morris, Richard; Karenowska, Alexy

    Propagating microwave-frequency magnons in magnetic films attract increasing attention on account of their potential interface with superconducting quantum circuit and qubit systems. Their rich dynamics and slow speeds make magnons an interesting addition to the circuit quantum electrodynamics toolbox and, at the same time, superconducting circuit technology promises to be a powerful tool in the investigation of their quantum properties. We have studied the propagation of pulsed surface spin-wave signals over millimeter distances in yttrium iron garnet waveguides at ~ 10 mK . Input microwave pulses and pulse trains with various envelope shapes were applied to an inductive input antenna, and the resulting magnons were detected by an output antenna of identical design. The shape of the output signal was observed to depend on the frequency content (carrier and pulse shape) of the input pulse. By performing measurements at varying frequencies and magnetic fields we have been able to map out the dispersion relation for surface magnon modes. These experiments were undertaken as a first step towards coupling propagating magnons in thin films to other quantum systems with microwave-frequency transition energies, and superconducting qubits in particular. The authors acknowledge support from the EPSRC (EP/K032690/1).

  6. Laser-induced periodic surface structures nanofabricated on poly(trimethylene terephthalate) spin-coated films.

    Science.gov (United States)

    Martín-Fabiani, I; Rebollar, E; Pérez, S; Rueda, D R; García-Gutiérrez, M C; Szymczyk, A; Roslaniec, Z; Castillejo, M; Ezquerra, T A

    2012-05-22

    Here we present a precise morphological description of laser-induced periodic surface structures (LIPSS) nanofabricated on spin-coated poly(trimethylene terephthalate) (PTT) films by irradiation with 266 nm, 6 ns laser pulses and by using a broad range of fluences and number of pulses. By accomplishing real and reciprocal space measurements by means of atomic force microscopy and grazing incidence wide- and small-angle X-ray scattering respectively on LIPSS samples, the range of optimum structural order has been established. For a given fluence, an increase in the number of pulses tends to improve LIPSS in PTT. However, as the pulse doses increase above a certain limit, a distortion of the structures is observed and a droplet-like morphology appears. It is proposed that this effect could be related to a plausible decrease of the molecular weight of PTT due to laser-induced chain photo-oxidation by irradiation with a high number of pulses. A concurrent decrease in viscosity enables destabilization of LIPSS by the formation of droplets in a process similar to surface-limited dewetting.

  7. Identifying and tracing potential energy surfaces of electronic excitations with specific character via their transition origins: application to oxirane.

    Science.gov (United States)

    Li, Jian-Hao; Zuehlsdorff, T J; Payne, M C; Hine, N D M

    2015-05-14

    We show that the transition origins of electronic excitations identified by quantified natural transition orbital (QNTO) analysis can be employed to connect potential energy surfaces (PESs) according to their character across a wide range of molecular geometries. This is achieved by locating the switching of transition origins of adiabatic potential surfaces as the geometry changes. The transition vectors for analysing transition origins are provided by linear response time-dependent density functional theory (TDDFT) calculations under the Tamm-Dancoff approximation. We study the photochemical CO ring opening of oxirane as an example and show that the results corroborate the traditional Gomer-Noyes mechanism derived experimentally. The knowledge of specific states for the reaction also agrees well with that given by previous theoretical work using TDDFT surface-hopping dynamics that was validated by high-quality quantum Monte Carlo calculations. We also show that QNTO can be useful for considerably larger and more complex systems: by projecting the excitations to those of a reference oxirane molecule, the approach is able to identify and analyse specific excitations of a trans-2,3-diphenyloxirane molecule.

  8. Coherence and Decoherence of a Localized Excitation on a Surface Adatom

    Institute of Scientific and Technical Information of China (English)

    高世武; H.Petek; J.Aizpurua; P.Apell

    2002-01-01

    A theory of coherent excitation of a localized state on an adatom by two-photon photoemission spectroscopy(TR-2PPE) is presented within a microscopic model and the time-dependent formalism. Coherent oscillation and incoherent population decay of the excitation are obtained, and are shown to attain well-defined lifetime constants only in the long-delay limit. In addition, we have found a competing excitation channel via electron transfer. The theory is applied to Cs/Cu (111), which reproduces a few qualitative features observed in recent experiments. The effect of atomic motion on the 2PPE spectra, which manifests dominantly as a redshift in the spectrum, has been analysed.

  9. 1300 nm optically pumped quantum dot spin vertical external-cavity surface-emitting laser

    Energy Technology Data Exchange (ETDEWEB)

    Alharthi, S. S., E-mail: ssmalh@essex.ac.uk; Henning, I. D.; Adams, M. J. [School of Computer Science and Electronic Engineering, University of Essex, Wivenhoe Park, Colchester CO4 3SQ (United Kingdom); Orchard, J. [Department of Physics and Astronomy, University of Sheffield, Hounsfield Road, Sheffield S3 7RH (United Kingdom); Clarke, E. [EPSRC National Centre for III-V Technologies, University of Sheffield, Mappin Street, S1 3JD Sheffield (United Kingdom)

    2015-10-12

    We report a room temperature optically pumped Quantum Dot-based Spin-Vertical-External-Cavity Surface-Emitting laser (QD Spin-VECSEL) operating at the telecom wavelength of 1.3 μm. The active medium was composed of 5 × 3 QD layers; each threefold group was positioned at an antinode of the standing wave of the optical field. Circularly polarized lasing in the QD-VECSEL under Continuous-Wave optical pumping has been realized with a threshold pump power of 11 mW. We further demonstrate at room temperature control of the QD-VECSEL output polarization ellipticity via the pump polarization.

  10. Effect of Catch Cup Geometry on 3D Boundary Layer Flow over the Wafer Surface in a Spin Coating

    Institute of Scientific and Technical Information of China (English)

    Mizue MUNEKATA; Seiichi KIMURA; Hiroaki KURISHIMA; Jinsuke TANAKA; Sohei YAMAMOTO; Hiroyuki YOSHIKAWA; Kazuyoshi MATSUZAKI; Hideki OHBA

    2008-01-01

    Recently, development of high technology has been required for the formation of thin uniform fdm in manufacturing processes of semiconductor as the semiconductor instruments become more sophisticated. Spin coating is usually used for spreading photoresist on a wafer surface. However, since rotating speed of the disk is very high in spin coating, the dropped photoresist scatters outward and reattaches on the film surface. A catch cup is set up outside the wafer in spin coating, and scattered photoresist mist is removed from the wafer edge by the exhaust flow generated at the gap between the wafer edge and the catch cup. In the dry process of a spin coating, it is a serious concern that the film thickness increases near the wafer edge in the case of low rotating speed. The purpose of this study is to make clear the effect of the catch cup geometry on the 3D boundary layer flow over the wafer surface and the drying rate of liquid film.

  11. Fermi Surface of Sr_{2}RuO_{4}: Spin-Orbit and Anisotropic Coulomb Interaction Effects.

    Science.gov (United States)

    Zhang, Guoren; Gorelov, Evgeny; Sarvestani, Esmaeel; Pavarini, Eva

    2016-03-11

    The topology of the Fermi surface of Sr_{2}RuO_{4} is well described by local-density approximation calculations with spin-orbit interaction, but the relative size of its different sheets is not. By accounting for many-body effects via dynamical mean-field theory, we show that the standard isotropic Coulomb interaction alone worsens or does not correct this discrepancy. In order to reproduce experiments, it is essential to account for the Coulomb anisotropy. The latter is small but has strong effects; it competes with the Coulomb-enhanced spin-orbit coupling and the isotropic Coulomb term in determining the Fermi surface shape. Its effects are likely sizable in other correlated multiorbital systems. In addition, we find that the low-energy self-energy matrix-responsible for the reshaping of the Fermi surface-sizably differs from the static Hartree-Fock limit. Finally, we find a strong spin-orbital entanglement; this supports the view that the conventional description of Cooper pairs via factorized spin and orbital part might not apply to Sr_{2}RuO_{4}.

  12. Spin Hall effects in metallic multilayers (Conference Presentation)

    Science.gov (United States)

    Woltersdorf, Georg; Wei, Dahai H.; Obstbaum, Martin; Back, Christian H.; Decker, Martin

    2016-10-01

    We study the direct as well as the inverse SHE. In the case of the direct SHE a dc charge current is applied in the plane of a ferromagnet/normal metal layer stack and the SHE creates a spin polarization at the surface of the normal metal leading to the injection of a spin current into the ferromagnet. This spin current is absorbed in the ferromagnet and causes a spin transfer torque. Using time and spatially resolved Kerr microscopy we measure the transferred spin momentum and compute the spin Hall angle. In a second set of experiments using identical samples pure spin currents are injected by the spin pumping effect from the ferromagnet into the normal metal. The spin current injected by spin pumping has a large ac component transverse to the static magnetization direction and a very small dc component parallel to the magnetization direction. The inverse SHE converts these spin current into charge current. The corresponding inverse SHE voltages induced by spin pumping at ferromagnetic resonance are measured in permalloy/platinum and permalloy/gold multilayers in various excitation geometries and as a function of frequency in order to separate the contributions of anisotropic magnetoresistance and SHE. In addition, we present experimental evidence for the ac component of inverse SHE voltages generated by spin pumping.

  13. Control on wetting properties of spin-deposited silica films by surface silylation method

    Energy Technology Data Exchange (ETDEWEB)

    Rao, A. Venkateswara, E-mail: avrao2012@gmail.com [Air Glass Laboratory, Department of Physics, Shivaji University, Kolhapur 416 004, Maharashtra (India); Latthe, Sanjay S.; Dhere, Sunetra L.; Pawar, Swapnali S. [Air Glass Laboratory, Department of Physics, Shivaji University, Kolhapur 416 004, Maharashtra (India); Imai, Hiroaki [Faculty of Science and Technology, Keio University, 3-14-1 Hiyoshi, Kohoku-ku, Yokohama 223-8522 (Japan); Ganesan, V. [CSR, Indore Centre, University Campus, Khandwa Road, Indore 452 017, Madhyapradesh (India); Gupta, Satish C.; Wagh, Pratap B. [Applied Physics Division, Bhabha Atomic Research Centre (BARC), Trombay, Mumbai 400 085 (India)

    2010-01-15

    Control on the wettability of solid materials by liquid is a classical and key issue in surface engineering. Optically transparent water-repellent silica films have been spin-deposited on glass substrates at room temperature ({approx}27 deg. C). The wetting behavior of silica films was controlled by surface silylation method using dimethylchlorosilane (DMCS) as a silylating reagent. A coating sol was prepared by keeping the molar ratio of methyltrimethoxysilane (MTMS) precursor, methanol (MeOH) solvent, water (H{sub 2}O) constant at 1:8.8:2.64 respectively, with 4 M NH{sub 4}OH as a catalyst throughout the experiments and the amount of DMCS in hexane was varied from 0 to 12 vol.%. It was found that with an increase in vol.% of DMCS, the water contact angle values of the films increased from 78 deg. to 136 deg. At 12 vol.% of DMCS, the film shows static water contact angle as high as 136 deg. and water sliding angle as low as 18 deg. The hydrophobic silica films retained their water repellency up to a temperature 295 deg. C and above this temperature the films show superhydrophilic behavior. These results are compared with our earlier research work done on silylation of silica surface using hexamethyldisilazane (HMDZ) and trimethylchlorosilane (TMCS). The hydrophobic silica films were characterized by taking into consideration the Fourier transform infrared (FT-IR) spectroscopy, thermo gravimetric-differential thermal (TG-DT) analyses, scanning electron microscopy (SEM), atomic force microscopy (AFM), % of optical transmission, thermal and chemical aging tests, humidity tests, static and dynamic water contact angle measurements.

  14. Control on wetting properties of spin-deposited silica films by surface silylation method

    Science.gov (United States)

    Rao, A. Venkateswara; Latthe, Sanjay S.; Dhere, Sunetra L.; Pawar, Swapnali S.; Imai, Hiroaki; Ganesan, V.; Gupta, Satish C.; Wagh, Pratap B.

    2010-01-01

    Control on the wettability of solid materials by liquid is a classical and key issue in surface engineering. Optically transparent water-repellent silica films have been spin-deposited on glass substrates at room temperature (˜27 °C). The wetting behavior of silica films was controlled by surface silylation method using dimethylchlorosilane (DMCS) as a silylating reagent. A coating sol was prepared by keeping the molar ratio of methyltrimethoxysilane (MTMS) precursor, methanol (MeOH) solvent, water (H 2O) constant at 1:8.8:2.64 respectively, with 4 M NH 4OH as a catalyst throughout the experiments and the amount of DMCS in hexane was varied from 0 to 12 vol.%. It was found that with an increase in vol.% of DMCS, the water contact angle values of the films increased from 78° to 136°. At 12 vol.% of DMCS, the film shows static water contact angle as high as 136° and water sliding angle as low as 18°. The hydrophobic silica films retained their water repellency up to a temperature 295 °C and above this temperature the films show superhydrophilic behavior. These results are compared with our earlier research work done on silylation of silica surface using hexamethyldisilazane (HMDZ) and trimethylchlorosilane (TMCS). The hydrophobic silica films were characterized by taking into consideration the Fourier transform infrared (FT-IR) spectroscopy, thermo gravimetric-differential thermal (TG-DT) analyses, scanning electron microscopy (SEM), atomic force microscopy (AFM), % of optical transmission, thermal and chemical aging tests, humidity tests, static and dynamic water contact angle measurements.

  15. Study of natural spin-parity strange meson radial excitations in K/sup -/p. -->. K/sup -/. pi. /sup +/n at 11 GeV/c

    Energy Technology Data Exchange (ETDEWEB)

    Durkin, L.S.

    1980-12-01

    Results are presented from a high statistics study of the reaction K/sup -/p ..-->.. K/sup -/..pi../sup +/n at 11 GeV/c. This data was selected offline from an approx. 1000 event/..mu..b K/sup -/p experiment run on the Large Aperture Solenoid Spectrometer (LASS) at SLAC which triggered on essentially the total inelastic cross section. This K/sup -/..pi../sup +/n sample, after cuts, contained approx. 42,000 events in the K..pi.. invariant mass region from 0.65 GeV to 2.30 GeV, and absolute value t' < 0.2 GeV/sup 2/. A spherical harmonic angular moments analysis of this data is presented, as well as an energy independent partial wave analysis (PWA) of these angular moments. The nearly uniform acceptance characteristics of this data allowed a detailed analysis, which yielded information on natural spin-parity strange meson resonances in the K..pi.. invariant mass range from 0.65 GeV to 2.30 GeV. The well established K*(895), K*(1430), and K*(1780) are observed, and clear evidence is presented for a J/sup P/ = 4/sup +/ strange meson state at a mass of 2.08 GeV. The K/sup -/..pi../sup +/ elastic scattering partial waves extracted in this PWA show unambiguous evidence for a relatively narrow S wave resonance near 1.42 GeV in the K..pi.. invariant mass. This state is a confirmation of the 0/sup +/ K(1500) seen in previous PWA's. A new higher S wave resonance is clearly seen unambiguously near 1.90 GeV. Unambiguous evidence is presented for a relatively wide P wave resonance in the 1.70 GeV region.A second new P wave resonance also is seen in two of four ambiguous partial wave solutions in the 2.10 GeV region. These resonance states are discussed within the framework of a simple harmonic oscillator quark model. In particular three of the underlying resonances are discussed as possible natural spin-parity strange meson radial excitations.

  16. Circular polarization switching and bistability in an optically injected 1300 nm spin-vertical cavity surface emitting laser

    Energy Technology Data Exchange (ETDEWEB)

    Alharthi, S. S., E-mail: ssmalh@essex.ac.uk; Henning, I. D.; Adams, M. J. [School of Computer Science and Electronic Engineering, University of Essex, Wivenhoe Park, Colchester CO4 3SQ (United Kingdom); Hurtado, A. [School of Computer Science and Electronic Engineering, University of Essex, Wivenhoe Park, Colchester CO4 3SQ (United Kingdom); Institute of Photonics, Physics Department, University of Strathclyde, Wolfson Centre, 106 Rottenrow East, Glasgow G4 0NW, Scotland (United Kingdom); Korpijarvi, V.-M.; Guina, M. [Optoelectronics Research Centre (ORC), Tampere University of Technology, P.O. Box 692, FIN-33101 Tampere (Finland)

    2015-01-12

    We report the experimental observation of circular polarization switching (PS) and polarization bistability (PB) in a 1300 nm dilute nitride spin-vertical cavity surface emitting laser (VCSEL). We demonstrate that the circularly polarized optical signal at 1300 nm can gradually or abruptly switch the polarization ellipticity of the spin-VCSEL from right-to-left circular polarization and vice versa. Moreover, different forms of PS and PB between right- and left-circular polarizations are observed by controlling the injection strength and the initial wavelength detuning. These results obtained at the telecom wavelength of 1300 nm open the door for novel uses of spin-VCSELs in polarization sensitive applications in future optical systems.

  17. Surface spin-glass, large surface anisotropy, and depression of magnetocaloric effect in La0.8Ca0.2MnO3 nanoparticles

    Science.gov (United States)

    Xi, S. B.; Lu, W. J.; Wu, H. Y.; Tong, P.; Sun, Y. P.

    2012-01-01

    The surface magnetic behavior of La0.8Ca0.2MnO3 nanoparticles was investigated. We observed irreversibility in high magnetic field. The surface spin-glass behavior as well as the high-field irreversibility is suppressed by increasing particle size while the freezing temperature TF does not change with particle size. The enhanced coercivity has been observed in the particles and we attributed it to the large surface anisotropy. We have disclosed a clear relationship between the particle size, the thickness of the shell, and the saturation magnetization of the particles. The large reduction of the saturation magnetization of the samples is found to be induced by the increase of nonmagnetic surface large since the thickness of the spin-disordered surface layer increases with a decrease in the particle size. Due to the reduction of the magnetization, the magnetocaloric effect (MCE) has been reduced by the decreased particle size since the nonmagnetic surface contributes little to the MCE. Based on the core-shell structure, large relative cooling powers RCP(s) of 180 J/kg and 471 J/kg were predicted for a field change of 2.0 T and 4.5 T, respectively, in the small particles with thin spin-glass layer. PMID:23319829

  18. Surface spin-glass, large surface anisotropy, and depression of magnetocaloric effect in La(0.8)Ca(0.2)MnO(3) nanoparticles.

    Science.gov (United States)

    Xi, S B; Lu, W J; Wu, H Y; Tong, P; Sun, Y P

    2012-12-15

    The surface magnetic behavior of La(0.8)Ca(0.2)MnO(3) nanoparticles was investigated. We observed irreversibility in high magnetic field. The surface spin-glass behavior as well as the high-field irreversibility is suppressed by increasing particle size while the freezing temperature T(F) does not change with particle size. The enhanced coercivity has been observed in the particles and we attributed it to the large surface anisotropy. We have disclosed a clear relationship between the particle size, the thickness of the shell, and the saturation magnetization of the particles. The large reduction of the saturation magnetization of the samples is found to be induced by the increase of nonmagnetic surface large since the thickness of the spin-disordered surface layer increases with a decrease in the particle size. Due to the reduction of the magnetization, the magnetocaloric effect (MCE) has been reduced by the decreased particle size since the nonmagnetic surface contributes little to the MCE. Based on the core-shell structure, large relative cooling powers RCP(s) of 180 J/kg and 471 J/kg were predicted for a field change of 2.0 T and 4.5 T, respectively, in the small particles with thin spin-glass layer.

  19. Electron doping evolution of the magnetic excitations in NaFe1 -xCoxAs

    Science.gov (United States)

    Carr, Scott V.; Zhang, Chenglin; Song, Yu; Tan, Guotai; Li, Yu; Abernathy, D. L.; Stone, M. B.; Granroth, G. E.; Perring, T. G.; Dai, Pengcheng

    2016-06-01

    We use time-of-flight (TOF) inelastic-neutron-scattering (INS) spectroscopy to investigate the doping dependence of magnetic excitations across the phase diagram of NaFe1 -xCoxAs with x =0 , 0.0175, 0.0215, 0.05, and 0.11 . The effect of electron doping by partially substituting Fe by Co is to form resonances that couple with superconductivity, broaden, and suppress low-energy (E ≤80 meV) spin excitations compared with spin waves in undoped NaFeAs. However, high-energy (E >80 meV) spin excitations are weakly Co-doping-dependent. Integration of the local spin dynamic susceptibility χ''(ω ) of NaFe1 -xCoxAs reveals a total fluctuating moment of 3.6 μB2/Fe and a small but systematic reduction with electron doping. The presence of a large spin gap in Co-overdoped nonsuperconducting NaFe0.89Co0.11As suggests that Fermi surface nesting is responsible for low-energy spin excitations. These results parallel the Ni-doping evolution of spin excitations in BaFe2 -xNixAs2 in spite of the differences in crystal structures and Fermi surface evolution in these two families of iron pnictides, thus confirming the notion that low-energy spin excitations coupling with itinerant electrons are important for superconductivity, while weakly doping-dependent high-energy spin excitations result from localized moments.

  20. Plasmon switching: observation of dynamic surface plasmon steering by selective mode excitation in a sub-wavelength slit.

    Science.gov (United States)

    Raghunathan, S B; Gan, C H; van Dijk, T; Ea Kim, B; Schouten, H F; Ubachs, W; Lalanne, P; Visser, T D

    2012-07-02

    We report a plasmon steering method that enables us to dynamically control the direction of surface plasmons generated by a two-mode slit in a thin metal film. By varying the phase between different coherent beams that are incident on the slit, individual waveguide modes are excited. Different linear combinations of the two modes lead to different diffracted fields at the exit of the slit. As a result, the direction in which surface plasmons are launched can be controlled. Experiments confirm that it is possible to distribute an approximately constant surface plasmon intensity in any desired proportion over the two launching directions. We also find that the anti-symmetric mode generates surface plasmons more efficiently than the fundamental symmetric mode.