Assay of low-enriched uranium using spontaneous fission neutrons
International Nuclear Information System (INIS)
Zucker, M.S.; Fainberg, A.
1980-01-01
Low-enriched uranium oxide in bulk containers can be assayed for safeguards purposes, using the neutrons from spontaneous fission of 238 U as a signature, to complement enrichment and mass measurement. The penetrability of the fast fission neutrons allows the inner portion of bulk samples to register. The measurement may also be useful for measuring moisture content, of significance in process control. The apparatus used can be the same as for neutron correlation counting for Pu assay. The neutron multiplication observed in 238 U is of intrinsic interest
Ternary fission of spontaneously fissile uranium isomers excited by neutrons
International Nuclear Information System (INIS)
Makarenko, V.E.; Molchanov, Y.D.; Otroshchenko, G.A.; Yan'kov, G.B.
1989-01-01
Spontaneously fissile isomers (SFI) of uranium were excited in the reactions 236,238 U(n,n') at an average neutron energy 4.5 MeV. A pulsed electrostatic accelerator and time analysis of the fission events were used. Fission fragments were detected by the scintillation method, and long-range particles from fission were detected by an ionization method. The relative probability of fission of nuclei through a spontaneously fissile isomeric state was measured: (1.30±0.01)·10 -4 ( 236 U) and (1.48±0.02)·10 -4 ( 238 U). Half-lives of the isomers were determined: 121±2 nsec (the SFI 236 U) and 267±13 nsec (the SFI 238 U). In study of the ternary fission of spontaneously fissile isotopes of uranium it was established that the probability of the process amounts to one ternary fission per 163±44 binary fissions of the SFI 236 U and one ternary fission per 49±14 binary fissions of the SFI 238 U. The substantial increase of the probability of ternary fission of SFI of uranium in comparison with the case of ternary fission of nuclei which are not in an isomeric state may be related to a special nucleon configuration of the fissile isomers of uranium
Prompt neutron spectrum of the spontaneous fission of californium-252
International Nuclear Information System (INIS)
Zamyatnin, Yu.S.; Kroshkin, N.I.; Korostylev, V.A.; Nefedov, V.N.; Ryazanov, D.K.; Starostov, B.I.; Semenov, A.F.
1976-01-01
The californium-252 spontaneous fission neutron spectrum was measured in the energy range of 0.01 to 10 MeV by the time-of-flight technique using various neutron detectors. The measurements of 252 Cf neutron spectrum at energies of 0.01 to 5 MeV were performed as a function of fission fragment kinetic energy. The mean neutron spectrum energy in the range of 0.7 to 10 MeV was found from the results of measurements. The irregularity in the 252 Cf neutron spectrum in the neutron energy range of less than 0.7 MeV compared to theoretical values is discussed. The mechanism of 252 Cf neutron emission is also discussed on the basis of neutron yield angle measurements. 12 references
Neutron detector for detecting rare events of spontaneous fission
International Nuclear Information System (INIS)
Ter-Akop'yan, G.M.; Popeko, A.G.; Sokol, E.A.; Chelnokov, L.P.; Smirnov, V.I.; Gorshkov, V.A.
1981-01-01
The neutron detector for registering rare events of spontaneous fission by detecting multiple neutron emission is described. The detector represents a block of plexiglas of 550 mm diameter and 700 mm height in the centre of which there is a through 160 mm diameter channel for the sample under investigation. The detector comprises 56 3 He filled counters (up to 7 atm pressure) with 1% CO 2 addition. The counters have a 500 mm length and a 32 mm diameter. The sampling of fission events is realized by an electron system which allows determining the number of detected neutrons, numbers of operated counters, signal amplitude and time for fission event detecting. A block diagram of a neutron detector electron system is presented and its operation principle is considered. For protection against cosmic radiation the detector is surronded by a system of plastic scintillators and placed behind the concrete shield of 6 m thickness. The results of measurements of background radiation are given. It has been found that the background radiation of single neutron constitutes about 150 counts per hour, the detecting efficiency of single neutron equals 0.483 +- 0.005, for a 10l detector sensitive volume. By means of the detector described the parameters of multiplicity distribution of prompt neutrons for 256 Fm spontaneous fission are measured. The average multiplicity equals 3.59+-0.06 the dispersion being 2.30+-0.65
Yields of correlated fragment pairs and neutron multiplicity in spontaneous fission of {sup 242}Pu
Energy Technology Data Exchange (ETDEWEB)
Veselsky, M.; Kliman, J.; Morhaccaron, M. [Institute of Physics of Slovak Academy of Sciences, Dubravska 9, 84228 Bratislava (Slovakia); Ramayya, A.V.; Kormicki, J.; Daniel, A.V. [Physics Department, Vanderbilt University, Nashville (United States)] Rasmussen, J.O. [Lawrence Berkeley National Laboratory, Berkeley (United States)] Stoyer, M.A. [Lawrence Livermore National Laboratory, Livermore (United States); Daniel, A.V.; Popeko, G.S.; Oganessian, Yu. Ts. [Joint Institute for Nuclear Research, Dubna (Russia)] Greiner, W. [Institut fur Theoretische Physik, J. W. Goethe Universitaet, Frankfurt a. M. (Germany); Aryaeinejad, R. [Idaho National Engineering Laboratory, Idaho Falls (United States)
1998-10-01
Yields of correlated fragment pairs were obtained in spontaneous fission of {sup 242}Pu. Charge, mass and neutron multiplicity distributions of fragment pairs were determined and compared to available data. The yield of cold fission without neutron emission was determined to about 10{percent} for the set of observed correlated fragment pairs. {copyright} {ital 1998 American Institute of Physics.}
The measurement of prompt neutron spectrum in spontaneous fission of {sup 244}Cm
Energy Technology Data Exchange (ETDEWEB)
Batenkov, O.I.; Boykov, G.S.; Drapchinsky, L.V.; Majorov, M.Ju.; Trenkin, V.A. [V.G. Khlopin Radium Inst., Saint Petersburg (Russian Federation)
1997-03-01
Under the Program of Measurements of Prompt Fission Neutron Spectra of Minor Actinides for Transmutation Purposes the integral neutron spectrum in spontaneous fission of {sup 244}Cm has been measured by the time-of-flight method in the energy range of 0.1-15 MeV relative to the standard neutron spectrum in {sup 252}Cf spontaneous fission. Essential attention was paid to revealing of possible systematic errors. It is shown, that the {sup 244}Cm spectrum shape may be well described by using Mannhart evaluation with appropriate parameter of Maxwell temperature T{sub M} = 1.37 MeV. (author)
Neutron-neutron angular correlations in spontaneous fission of 252Cf and 240Pu
Verbeke, J. M.; Nakae, L. F.; Vogt, R.
2018-04-01
Background: Angular anisotropy has been observed between prompt neutrons emitted during the fission process. Such an anisotropy arises because the emitted neutrons are boosted along the direction of the parent fragment. Purpose: To measure the neutron-neutron angular correlations from the spontaneous fission of 252Cf and 240Pu oxide samples using a liquid scintillator array capable of pulse-shape discrimination. To compare these correlations to simulations combining the Monte Carlo radiation transport code MCNPX with the fission event generator FREYA. Method: Two different analysis methods were used to study the neutron-neutron correlations with varying energy thresholds. The first is based on setting a light output threshold while the second imposes a time-of-flight cutoff. The second method has the advantage of being truly detector independent. Results: The neutron-neutron correlation modeled by FREYA depends strongly on the sharing of the excitation energy between the two fragments. The measured asymmetry enabled us to adjust the FREYA parameter x in 240Pu, which controls the energy partition between the fragments and is so far inaccessible in other measurements. The 240Pu data in this analysis was the first available to quantify the energy partition for this isotope. The agreement between data and simulation is overall very good for 252Cf(sf ) and 240Pu(sf ) . Conclusions: The asymmetry in the measured neutron-neutron angular distributions can be predicted by FREYA. The shape of the correlation function depends on how the excitation energy is partitioned between the two fission fragments. Experimental data suggest that the lighter fragment is disproportionately excited.
Correlation studies of neutron multiplicities in the 252Cf spontaneous fission
International Nuclear Information System (INIS)
Alkhazov, I.D.; Dmitriev, V.D.; Kovalenko, S.S.; Kuznetsov, A.V.; Malkin, L.Z.; Petrzhak, K.A.; Petrov, B.F.; Shpakov, V.I.
1988-01-01
Correlations between the numbers of neutrons emitted by the 252 Cf spontaneous fission fragments have been studied as a function of the fragment mass and total kinetic energy. Behaviour of the neutron number dispersions and covariances was studied for the region of symmetric fission. Parameters of the complementary fragment excitation energy distribution (mean values, dispersions, covariances) were determined. Various factors describing correlations between the complementary fragment excitation energies are considered
Prompt neutron energy spectrum for the spontaneous fission of Cf-252
International Nuclear Information System (INIS)
Blinov, M.V.; Boykov, G.S.; Vitenko, V.A.
1985-06-01
The prompt neutron spectrum for the spontaneous fission of Cf-252 has been measured in 0.01-10 MeV region by the time-of-flight technique using a fast ionization chamber with U-235 layers as the neutron detector. Numerical data for the spectrum are presented, with an error file. (author)
An evaluation of the spontaneous fission prompt neutron spectrum of 252Cf
International Nuclear Information System (INIS)
Bojkov, G.S.; Yurevich, V.I.
1987-01-01
An evaluation of the spontaneous fission prompt neutron spectrum of 252 Cf from 1 keV to 20 MeV is described. Variance-covariance matrices for a number of recent experimental data sets were constructed and used to evaluate the neutron spectrum following a Bayesian procedure. The evaluated spectrum is compared with various experimental and theoretical representations. (author)
Energy Technology Data Exchange (ETDEWEB)
Shanglian, Bao; Jinquan, Liu [Beijing Univ., BJ (China); Batenkov, O I; Blinov, M V; Smirnov, S N [V.G. Khlopin Radium Institute, ST. Petersburg (Russian Federation)
1994-09-01
The {sup 252}Cf spontaneous prompt fission neutron spectrum at 0 degree and 180 degree relative to the motion direction of corresponding fission fragments was measured. High angular resolution for fragment measurements and high energy resolution for neutron measurements were obtained using multi-parameter TOF spectrometer. The results showed that there is a symmetric distribution of `forward` and `backward` for low energy in C.M.S. neutrons, which was an evidence of nonequilibrium neutrons existed in fission process.
Energy and angular distributions of neutrons from 252Cf spontaneous fission
International Nuclear Information System (INIS)
Vasil'ev, Yu.A.; Sidorov, L.V.; Vasil'eva, N.K.
1982-01-01
Some results from a first series of measurements of energy and angular distributions of neutrons from 252 Cf spontaneous fission using a spectrometer with high neutron detection efficiency, i.e. a 4π neutron time-of-flight spectrometer, were already presented. Subsequently, a second series of measurements was performed using a more sophisticated technique. For this second series, we used a more intense 252 Cf layer (25,000 spontaneous fissions per second). The angular resolution was improved by a factor of 2-3 by combining the hexahedral counter modules, placed at the same angle with respect to the direction of motion of the fragments, in new panoramic counters. The neutron counters were calibrated against the average 252 Cf neutron spectrum at several positions of the axis of the fragment detector with respect to the neutron counters. In the spectrum measurements and calibration work, the scattered neutron background was not determined theoretically, as in the first series of measurements, but experimentally using four extra scintillation counters with scatter cones; the counters were set up at 60 deg., 80 deg., 100 deg., and 120 deg. to the direction of separation of the fragments
International Nuclear Information System (INIS)
Rodríguez-Guzmán, R; Robledo, L M
2017-01-01
Constrained mean-field calculations, based on the Gogny-D1M energy density functional, have been carried out to describe fission in Ra, U and Pu nuclei with neutron number 144 ≤ N ≤ 176. Fission paths, collective masses and zero-point quantum vibrational and rotational corrections are used to compute the spontaneous fission half-lives. We also pay attention to isomeric states along the considered fission paths. Alpha decay half-lives have also been computed using a parametrization of the Viola-Seaborg formula. Though there exists a strong variance of the predicted fission rates with respect to the details involved in their computation a robust trend is obtained indicating, that with increasing neutron number fission dominates over α -decay. Our results also suggest that a dynamical treatment of pairing correlations is required within the microscopic studies of the fission process in heavy nuclear systems. (paper)
International Nuclear Information System (INIS)
Perry, R.T.; Wilson, W.B.; Charlton, W.S.
1998-04-01
In many systems, it is imperative to have accurate knowledge of all significant sources of neutrons due to the decay of radionuclides. These sources can include neutrons resulting from the spontaneous fission of actinides, the interaction of actinide decay α-particles in (α,n) reactions with low- or medium-Z nuclides, and/or delayed neutrons from the fission products of actinides. Numerous systems exist in which these neutron sources could be important. These include, but are not limited to, clean and spent nuclear fuel (UO 2 , ThO 2 , MOX, etc.), enrichment plant operations (UF 6 , PuF 4 , etc.), waste tank studies, waste products in borosilicate glass or glass-ceramic mixtures, and weapons-grade plutonium in storage containers. SOURCES-3A is a computer code that determines neutron production rates and spectra from (α,n) reactions, spontaneous fission, and delayed neutron emission due to the decay of radionuclides in homogeneous media (i.e., a mixture of α-emitting source material and low-Z target material) and in interface problems (i.e., a slab of α-emitting source material in contact with a slab of low-Z target material). The code is also capable of calculating the neutron production rates due to (α,n) reactions induced by a monoenergetic beam of α-particles incident on a slab of target material. Spontaneous fission spectra are calculated with evaluated half-life, spontaneous fission branching, and Watt spectrum parameters for 43 actinides. The (α,n) spectra are calculated using an assumed isotropic angular distribution in the center-of-mass system with a library of 89 nuclide decay α-particle spectra, 24 sets of measured and/or evaluated (α,n) cross sections and product nuclide level branching fractions, and functional α-particle stopping cross sections for Z < 106. The delayed neutron spectra are taken from an evaluated library of 105 precursors. The code outputs the magnitude and spectra of the resultant neutron source. It also provides an
Energy Technology Data Exchange (ETDEWEB)
Gerasimenko, B.F. [V.G. Khlopin Radium Inst., Saint Peterburg (Russian Federation)
1997-03-01
The calculations of integral spectra of prompt neutrons of spontaneous fission of {sup 244}Cm and {sup 246}Cm were carried out. The calculations were done by the Statistical Computer Code Complex SCOFIN applying the Hauser-Feschbach method as applied to the description of the de-excitation of excited fission fragments by means of neutron emission. The emission of dipole gamma-quanta from these fragments was considered as a competing process. The average excitation energy of a fragment was calculated by two-spheroidal model of tangent fragments. The density of levels in an excited fragment was calculated by the Fermi-gas model. The quite satisfactory agreement was reached between theoretical and experimental results obtained in frames of Project measurements. The calculated values of average multiplicities of neutron number were 2,746 for {sup 244}Cm and 2,927 for {sup 246}Cm that was in a good accordance with published experimental figures. (author)
Neutron multiplicity of fission fragments
Energy Technology Data Exchange (ETDEWEB)
Abdelrahman, Y S [Physics department, mu` rah university Al-Karak, (Jordan)
1995-10-01
The total average neutron multiplicity of the fission fragments produced by the spontaneous fission of {sup 248} Cm has been measured. This measurement has been done by using a new experimental technique. This technique mainly depends on {gamma}-{gamma} coincidence using a very high resolution high purity germanium (HPGe) detector. 2 figs.
Prompt neutron emission from fragments in spontaneous fission of {sup 244,248}Cm and {sup 252}Cf
Energy Technology Data Exchange (ETDEWEB)
Vorobyev, A. S.; Shcherbakov, O. A. [Petersburg Nuclear Physics Institute, Gatchina, Leningrad district, 188300 (Russian Federation); Dushin, V. N.; Jakovlev, V. A.; Kalinin, V. A.; Petrov, B. F. [V.G. Khlopin Radium Institute, St. Petersburg, 194021 (Russian Federation); Hambsch, F.J [EC-JRC-Institute for Reference Materials and Measurements Retieseweg 111, B-2440 Geel (Belgium); Laptev, A. B. [Petersburg Nuclear Physics Institute, Gatchina, Leningrad district, 188300 (Russian Federation); Japan Nuclear Cycle Development Institute, Tokai-mura, Naka-gun, Ibaraki 319-1194 (Japan)
2005-07-01
Neutrons emitted in fission were measured separately for each complementary fragment in correlation with fission fragment energies. Two high efficiency Gd-loaded liquid scintillator tanks were used for neutron registration. Fission fragment energies were measured using a twin Frisch gridded ionization chamber with a pin-hole collimator. The neutron multiplicity distributions were obtained for each value of the fission fragment mass and energy and corrected for neutron registration efficiency, background and pile-up. The dependencies of these distributions on fragment mass and energy for different energy and mass bins, as well as the mass and energy distribution of the fission fragments are presented and discussed. (authors)
International Nuclear Information System (INIS)
Madland, D.G.; LaBauve, R.J.; Nix, J.R.
1984-01-01
Because of their importance as neutron standards, we present comparisons of measured and calculated prompt fission neutron spectra N(E) and average prompt neutron multiplicities anti nu/sub p/ for the spontaneous fission of 252 Cf. In particular, we test three representations of N(E) against recent experimental measurements of the differential spectrum and threshold integral cross sections. These representations are the Maxwellian spectrum, the NBS spectrum, and the Los Alamos spectrum of Madland and Nix. For the Maxwellian spectrum, we obtain the value of the Maxwellian temperature T/sub M/ by a least-squares adjustment to the experimental differential spectrum of Poenitz and Tamura. For the Los Alamos spectrum, a similar least-squares adjustment determines the nuclear level-density parameter a, which is the single unknown parameter that appears. The NBS spectrum has been previously constructed by adjustments to eight differential spectra measured during the period 1965 to 1974. Among these three representations, we find that the Los Alamos spectrum best reproduces both the differential and integral measurements, assuming ENDF/B-V cross sections in the calculation of the latter. Although the NBS spectrum reproduces the integral measurements fairly well, it fails to satisfactorily reproduce the new differential measurement, and the Maxwellian spectrum fails to satisfactorily reproduce the integral measurements. Additionally, we calculate a value of anti nu/sub p/ from the Los Alamos theory that is within approximately 1% of experiment. 25 references
Identification of new neutron-rich rare-earth nuclei produced in /sup 252/Cf spontaneous fission
Greenwood, R C; Gehrke, R J; Meikrantz, D H
1981-01-01
A program of systematic study of the decay properties of neutron-rich rare-earth nuclei with 30 s
Least squares analysis of fission neutron standard fields
International Nuclear Information System (INIS)
Griffin, P.J.; Williams, J.G.
1997-01-01
A least squares analysis of fission neutron standard fields has been performed using the latest dosimetry cross sections. Discrepant nuclear data are identified and adjusted spectra for 252 Cf spontaneous fission and 235 U thermal fission fields are presented
Fission neutron multiplicity calculations
International Nuclear Information System (INIS)
Maerten, H.; Ruben, A.; Seeliger, D.
1991-01-01
A model for calculating neutron multiplicities in nuclear fission is presented. It is based on the solution of the energy partition problem as function of mass asymmetry within a phenomenological approach including temperature-dependent microscopic energies. Nuclear structure effects on fragment de-excitation, which influence neutron multiplicities, are discussed. Temperature effects on microscopic energy play an important role in induced fission reactions. Calculated results are presented for various fission reactions induced by neutrons. Data cover the incident energy range 0-20 MeV, i.e. multiple chance fission is considered. (author). 28 refs, 13 figs
International Nuclear Information System (INIS)
Goldberg, H.J.; Morford, R.J.
1993-06-01
The disposal of high-level defense waste in a geologic repository necessitates conversion of the waste to a stable form. For this purpose, the Hanford Waste Vitrification Plant (HWVP) will be constructed. In this facility the waste will be converted into 6.3 x 10 5 cm 3 glassified cylinders, 59 cm in diameter and 230 cm in height, which will be placed in steel containers and buried. The waste packages must be adequately shielded to ensure the safety of personnel handling them. To calculate the shielding necessary, the radiation source term must be determined. Although the γ-ray source term does not present a problem, the neutron source term is a concern. Because the glass matrix is composed of light elements, the presence of any α-particle emitting radionuclides in the waste will contribute to the neutron flux. This paper attempts to ascertain the neutron flux and spectrum from (α,n) reactions and add it to the flux resulting from spontaneous fission
Spectroscopy of neutron-rich nuclei populated in the spontaneous fission of 252Cf and 248Cm
International Nuclear Information System (INIS)
Smith, A. G.; Simpson, G. S.; Billowes, J.; Durell, J. L.; Phillips, W. R.; Dagnall, P. J.; Freeman, S. J.; Leddy, M.; Roach, A. A.; Smith, J. F.
1999-01-01
In this paper we present research that has been carried out using the Euroball and Eurogam arrays to detect γ rays emitted from spontaneously fissioning 248 Cm and 252 Cf. The paper focuses on three sub-areas of current activity, namely, the measurement of yields of secondary fragment pairs, the measurement of state lifetimes at around spin 10, and recent measurements of g-factors of excited states in fission fragments. (c) 1999 American Institute of Physics
International Nuclear Information System (INIS)
Bessis, J.
1986-09-01
Methods are described for calculating the probabilities, p(m), of detection of m neutrons, inside a split millisecond counting gate, m varying from zero to some units. At the present stage, these methods suppose the source to be very small. Using the generating function concept, they concern both possible modes of the counting system, for opening gates, i.e.: 1) Trigger pulses randomly with regard to the emitted neutrons, 2) Trigger pulses from the detected neutrons themselves. Computed values are finally compared to the measured ones. This comparison seems to be very favourable, since the respective deviations are often lower than 1 % [fr
International Nuclear Information System (INIS)
Hulet, E.K.; Wild, J.F.; Lougheed, R.W.; Baisden, P.A.; Landrum, J.H.; Dougan, R.J.; Mustafa, M.; Ghiorso, A.; Nitschke, J.M.
1979-01-01
The mass and kinetic energy distributions of fission fragments from the spontaneous fission of th newly discovered nuclide 259 Md were obtained. 259 Md was identified as the E. C. daughter of 259 No, and was found to decay entirely (> 95%) by spontaneous fission with a 95-min half-life. From the kinetic energies measured for 397 pairs of coincident fragments, a mass distribution was derived that is symmetric with sigma = 13 amu. 259 Md, together with 258 Fm and 259 Fm, form a select group of three nuclides whose mass division in spontaneous fission is highly symmetric. Unlike the total-kinetic-energy (TKE) distributions of 258 Fm and 259 Fm, which peak at approx. = to 240 MeV, this distribution for 259 Md is broad and is 50 MeV lower in energy. Analysis of the mass and energy distributions shows that events near mass symmetry also exhibit a broad TKE distribution, with one-third of the symmetric events having TKEs less than 200 MeV. The associated of low TKEs with symmetric mass division in the fission of very heavy actinides is anomalous and inconsistent with theories based upon the emergence of fragment shells near the scission point. Either three-body fragmentation or peculiar fragment shapes are assumed as the cause for the large consumption of Coulomb energy observed for a significant fraction of symmetric fissions in 259 Md. 6 figures
International Nuclear Information System (INIS)
Starostov, B.I.; Semenov, A.F.; Nefedov, V.N.
1978-01-01
The measurement results on the prompt neutron spectra in 233 U, 235 U, 239 Pu thermal neutron fission in the energy range of 0.01-5 MeV and in 252 Cf spontaneous fission in the energy range of 0.01-10 MeV are presented. The time-of-flight method was used. The exceeding of the spectra over the Maxwell distributions is observed at E 252 Cf neutron fission spectra. The spectra analysis was performed after normalization of the spectra and corresponding Maxwell distributions for one and the same area. In the range of 0.05-0.22 MeV the yield of 235 U + nsub(t) fission neutrons is approximately 8 and approximately 15 % greater than the yield of 252 Cf and 239 Pu + nsub(t) fission neutrons, respectively. In the range of 0.3-1.2 MeV the yield of 235 U + nsub(t) fission neutrons is 8 % greater than the fission neutron yield in case of 239 Pu + nsub(t) fission. The 235 U + nsub(t) and 233 U + nsub(t) fission neutron spectra do not differ from one another in the 0.05-0.6 MeV range
Neutron emission during acceleration of 252Cf fission fragments
International Nuclear Information System (INIS)
Batenkov, O.I.; Blinov, M.V.; Blinov, A.B.; Smirnov, S.N.
1991-01-01
We investigate neutron emission during acceleration of fission fragments in the process of spontaneous fission of 252 Cf. Experimental angular and energy distributions of neutrons are compared with the results of calculations of neutron evaporation during fragment acceleration. (author). 8 refs, 3 figs
High-precision spectrometer for studies of ion-induced and spontaneous fission dynamics
International Nuclear Information System (INIS)
Batenkov, O.; Elmgren, K.; Majorov, M.; Blomgren, J.; Conde, H.; Hultqvist, S.; Olsson, N.; Rahm, J.; Ramstroem, E.; Smirnov, S.; Veshikov, A.
1997-01-01
A spectrometer has been designed and built to investigate the dynamics of spontaneous and ion-induced fission processes. It consists of 8 neutron detectors surrounding a low mass scattering chamber containing the fissionable targets and two fission fragment telescopes. The spectrometer measures neutron spectra, and energy and angular correlations of neutrons, as well as kinetic energy, mass, and relative angle of fission fragments. A 252 Cf fission reference source is used for calibration. (orig.)
Absolute calibration technique for spontaneous fission sources
International Nuclear Information System (INIS)
Zucker, M.S.; Karpf, E.
1984-01-01
An absolute calibration technique for a spontaneously fissioning nuclide (which involves no arbitrary parameters) allows unique determination of the detector efficiency for that nuclide, hence of the fission source strength
Nuclear data for neutron emission in the fission process
International Nuclear Information System (INIS)
Ganesan, S.
1991-11-01
This document contains the proceedings of the IAEA Consultants' Meeting on Nuclear Data for Neutron Emission in the Fission Process, Vienna, 22 - 24 October 1990. Included are the conclusions and recommendations reached at the meeting and the papers presented by the meeting participants. These papers provide a review of the status of experimental and theoretical data on neutron emission in spontaneous and neutron induced fission with reference to the data needs for reactor applications oriented towards actinide burner studies. The specific topics covered are the following: experimental measurements and theoretical predictions and evaluations of fission neutron energy spectra, average prompt fission neutron multiplicity, correlation in neutron emission from complementary fragments, neutron emission during acceleration of fission fragments, statistical properties of neutron rich nuclei by study of emission spectra of neutrons from the excited fission fragments, integral qualification of nu-bar for the major fissile isotopes, nu-bar total of 239 Pu and 235 U, and related problems. Refs figs and tabs
International Nuclear Information System (INIS)
Endo, A.; Sato, T.
2013-01-01
Absorbed doses, linear energy transfers (LETs) and quality factors of secondary charged particles in organs and tissues, generated via the interactions of the spontaneous fission neutrons from. 252 Cf and. 244 Pu within the human body, were studied using the Particle and Heavy Ion Transport Code System (PHITS) coupled with the ICRP Reference Phantom. Both the absorbed doses and the quality factors in target organs generally decrease with increasing distance from the source organ. The analysis of LET distributions of secondary charged particles led to the identification of the relationship between LET spectra and target-source organ locations. A comparison between human body-averaged mean quality factors and fluence-averaged radiation weighting factors showed that the current numerical conventions for the radiation weighting factors of neutrons, updated in ICRP103, and the quality factors for internal exposure are valid. (authors)
Fission fragment driven neutron source
Miller, Lowell G.; Young, Robert C.; Brugger, Robert M.
1976-01-01
Fissionable uranium formed into a foil is bombarded with thermal neutrons in the presence of deuterium-tritium gas. The resulting fission fragments impart energy to accelerate deuterium and tritium particles which in turn provide approximately 14 MeV neutrons by the reactions t(d,n).sup.4 He and d(t,n).sup.4 He.
New fission-neutron-spectrum representation for ENDF
International Nuclear Information System (INIS)
Madland, D.G.
1982-04-01
A new representation of the prompt fission neutron spectrum is proposed for use in the Evaluated Nuclear Data File (ENDF). The proposal is made because a new theory exists by which the spectrum can be accurately predicted as a function of the fissioning nucleus and its excitation energy. Thus, prompt fission neutron spectra can be calculated for cases where no measurements exist or where measurements are not possible. The mathematical formalism necessary for application of the new theory within ENDF is presented and discussed for neutron-induced fission and spontaneous fission. In the case of neutron-induced fission, expressions are given for the first-chance, second-chance, third-chance, and fourth-chance fission components of the spectrum together with that for the total spectrum. An ENDF format is proposed for the new fission spectrum representation, and an example of the use of the format is given
International Nuclear Information System (INIS)
Popkiewicz, M.; Osuch, S.; Szeflinski, Z.; Sztampke, A.; Wilhelmi, Z.; Wolinska, M.; Zaganczyk, R.
1997-01-01
The detection system MONA (Modular Neutron Array) consisting of eight large BC-501A liquid scintillators, was applied to determine the temperature of fission fragments emitted in spontaneous fission of 252 Cf. The determination of the temperature was based on the measurement of the neutron spectra
Energy Technology Data Exchange (ETDEWEB)
Popkiewicz, M.; Osuch, S.; Szeflinski, Z.; Sztampke, A.; Wilhelmi, Z.; Wolinska, M.; Zaganczyk, R. [Warsaw Univ., Inst. of Experimental Physics, Nuclear Physics Div., Warsaw (Poland)
1997-12-31
The detection system MONA (Modular Neutron Array) consisting of eight large BC-501A liquid scintillators, was applied to determine the temperature of fission fragments emitted in spontaneous fission of {sup 252}Cf. The determination of the temperature was based on the measurement of the neutron spectra. 5 refs, 2 figs.
Prompt fission neutron spectra and average prompt neutron multiplicities
International Nuclear Information System (INIS)
Madland, D.G.; Nix, J.R.
1983-01-01
We present a new method for calculating the prompt fission neutron spectrum N(E) and average prompt neutron multiplicity anti nu/sub p/ as functions of the fissioning nucleus and its excitation energy. The method is based on standard nuclear evaporation theory and takes into account (1) the motion of the fission fragments, (2) the distribution of fission-fragment residual nuclear temperature, (3) the energy dependence of the cross section sigma/sub c/ for the inverse process of compound-nucleus formation, and (4) the possibility of multiple-chance fission. We use a triangular distribution in residual nuclear temperature based on the Fermi-gas model. This leads to closed expressions for N(E) and anti nu/sub p/ when sigma/sub c/ is assumed constant and readily computed quadratures when the energy dependence of sigma/sub c/ is determined from an optical model. Neutron spectra and average multiplicities calculated with an energy-dependent cross section agree well with experimental data for the neutron-induced fission of 235 U and the spontaneous fission of 252 Cf. For the latter case, there are some significant inconsistencies between the experimental spectra that need to be resolved. 29 references
Mechanisms of fission neutron emission
International Nuclear Information System (INIS)
Maerten, H.
1991-01-01
The time evolution in fission is the starting point for discussing not only the main mechanism of fission neutron emission, the evaporation from fully accelerated fragments, but also possible secondary ones connected with dynamical features of nuclear fission. ''Asymptotic'' conditions as relevant for describing the particle release from highly excited, rapidly moving fragments are defined. Corresponding statistical model approaches to fission neutron emission, based on the adequate consideration of the intricate fragment occurrence probability, reproduce most of the experimental data. The remarkable influence of fission modes on neutron observables is analyzed in the framework of a macroscopic-microscopic scission point model consistent with energy conservation. Finally, chances and deficiencies for solving the mechanism puzzle are summarized. (author). 87 refs, 21 figs
Spontaneous fission of superheavy nuclei
Indian Academy of Sciences (India)
The fission-like configurations are used for the total deformation energy calculations. A ... oscillator potential for the two fission fragment regions reads as ... Beyond this limit, the contribution of more remote levels is negligible. Once the density ...
Insights into nuclear structure and the fission process from spontaneous fission
Energy Technology Data Exchange (ETDEWEB)
Hamilton, J.H.; Butler-Moore, K.; Ramayya, A.V. [Vanderbilt Univ., Nashville, TN (United States)] [and others
1993-12-31
The {gamma}-rays emitted following spontaneous and induced fission are rich sources of information about the structure of neutron-rich nuclei and about the fission process itself. The study of spontaneous fissioning isotopes with large Ge detector arrays are providing a wealth of such information as seen, for example, in recent reports. In this paper we present some of our most recent results on nuclear structure studies and conclusions on the fission process itself. In our work, we have employed in spontaneous fission, a triple gamma coincidence study for the first time and a high resolution, X-ray detector-{gamma}-coincidence study. These data provide powerful ways of separating the gamma rays which belong to a particular nucleus. The triple coincidence technique was used to uniquely identify the levels in {sup 136}Te and higher spin states in its N=84 isotones, {sup 138}Xe and {sup 140}Ba{sup 171}. Some other examples of the level structures observed in the low and high mass partners are presented, including a detailed analysis of the backbending of the moment of inertia in {sup 112,114,116}Pd. Finally, we present the first examples of how our analysis allows one to extract a detailed picture of the dependence of the angular momentum on the mass and atomic numbers of the fission fragments and of the long-sought neutron multiplicity distribution from zero-n to ten-n as a function of the charge and mass asymmetry.
Fission-neutrons source with fast neutron-emission timing
Energy Technology Data Exchange (ETDEWEB)
Rusev, G., E-mail: rusev@lanl.gov; Baramsai, B.; Bond, E.M.; Jandel, M.
2016-05-01
A neutron source with fast timing has been built to help with detector-response measurements. The source is based on the neutron emission from the spontaneous fission of {sup 252}Cf. The time is provided by registering the fission fragments in a layer of a thin scintillation film with a signal rise time of 1 ns. The scintillation light output is measured by two silicon photomultipliers with rise time of 0.5 ns. Overall time resolution of the source is 0.3 ns. Design of the source and test measurements using it are described. An example application of the source for determining the neutron/gamma pulse-shape discrimination by a stilbene crystal is given.
Post-scission fission theory: Neutron emission in fission
International Nuclear Information System (INIS)
Madland, D.G.
1997-01-01
A survey of theoretical representations of two of the observables in neutron emission in fission is given, namely, the prompt fission neutron spectrum N (E) and the average prompt neutron multiplicity bar ν p . Early representations of the two observables are presented and their deficiencies are discussed. This is followed by summaries and examples of recent theoretical models for the calculation of these quantities. Emphasis is placed upon the predictability and accuracy of the recent models. In particular, the dependencies of N (E) and bar ν p upon the fissioning nucleus and its excitation energy are treated. Recent work in the calculation of the prompt fission neutron spectrum matrix N (E, E n ), where E n is the energy of the neutron inducing fission, is then discussed. Concluding remarks address the current status of our ability to calculate these observables with confidence, the direction of future theoretical efforts, and limitations to current (and future) approaches
Nuclear fission and neutron-induced fission cross-sections
Energy Technology Data Exchange (ETDEWEB)
James, G.D.; Lynn, J.E.; Michaudon, A.; Rowlands, J.; de Saussure, G.
1981-01-01
A general presentation of current knowledge of the fission process is given with emphasis on the low energy fission of actinide nuclei and neutron induced fission. The need for and the required accuracy of fission cross section data in nuclear energy programs are discussed. A summary is given of the steps involved in fission cross section measurement and the range of available techniques. Methods of fission detection are described with emphasis on energy dependent changed and detector efficiency. Examples of cross section measurements are given and data reduction is discussed. The calculation of fission cross sections is discussed and relevant nuclear theory including the formation and decay of compound nuclei and energy level density is introduced. A description of a practical computation of fission cross sections is given.
Prompt neutron fission spectrum mean energies for the fissile nuclides and 252Cf
International Nuclear Information System (INIS)
Holden, N.E.
1985-01-01
The international standard for a neutron spectrum is that produced from the spontaneous fission of 252 Cf, while the thermal neutron induced fission neutron spectra for the four fissile nuclides, 233 U, 235 U, 239 Pu, and 241 Pu are of interest from the standpoint of nuclear reactors. The average neutron energies of these spectra are tabulated. The individual measurements are recorded with the neutron energy range measured, the method of detection as well as the average neutron energy for each author. Also tabulated are the measurements of the ratio of mean energies for pairs of fission neutron spectra. 75 refs., 9 tabs
On the mechanism of fission neutron emission
International Nuclear Information System (INIS)
Maerten, H.; Richter, D.; Seeliger, D.
1986-01-01
This review represents the present knowledge of the mechanism of prompt fission neutron emission. Starting with a brief fission process characterization related with neutron emission, possible emission mechanisms are discussed. It is emphasized that the experimental study of special mechanisms, i.e. scission neutron emission processes, requires a sufficiently correct description of emission probabilities on the base of the main mechanism, i.e. the evaporation from fully accelerated fragments. Adequate statistical-model approaches have to account for the complexity of nuclear fission reflected by an intricate fragment distribution. The present picture of scission neutron emission is not clarified neither experimentally nor theoretically. Deduced data are contradictory and depend on the used analysis procedures often involving rough discriptions of evaporated-neutron distributions. The contribution of two secondary mechanisms of fission neutron emission, i.e. the neutron evaporation during fragment acceleration and neutron emission due to the decay of 5 He after ternary fission, is estimated. We summarize the recent progress of the theoretical description of fission neutron spectra in the framework of statistical models considering the standard spectrum of 252 Cf(sf) neutrons especially. The main experimental basis for the study of fission neutron emission is the accurate measurement of emission probabilities as a function of emission energy and angle (at least) as well as fragment parameters (mass number ratio and kinetic energy). The present status is evaluated. (author)
Physics of neutron emission in fission
International Nuclear Information System (INIS)
Lemmel, H.D.
1989-06-01
The document contains the proceedings of the IAEA Consultants' Meeting on the Physics of Neutron Emission in Fission, Mito City (Japan), 24-27 May 1988. Included are the conclusions and recommendations reached at the meeting and the papers presented by the meeting participants. These papers cover the following topics: Energy dependence of the number of fission neutrons ν-bar (3 papers), multiplicity distribution of fission neutrons (3 papers), competition between neutron and γ-ray emission (4 papers), the fission neutron yield in resonances (2 papers) and the energy spectrum of fission neutrons in experiment (9 papers), theory (4 papers) and evaluation (1 paper). A separate abstract was prepared for each of these papers. Refs, figs and tabs
Status of measurements of fission neutron spectra of Minor Actinides
Energy Technology Data Exchange (ETDEWEB)
Drapchinsky, L.; Shiryaev, B. [V.G. Khlopin Radium Inst., Saint Petersburg (Russian Federation)
1997-03-01
The report considers experimental and theoretical works on studying the energy spectra of prompt neutrons emitted in spontaneous fission and neutron induced fission of Minor Actinides. It is noted that neutron spectra investigations were done for only a small number of such nuclei, most measurements, except those of Cf-252, having been carried out long ago by obsolete methods and imperfectapparatus. The works have no detailed description of experiments, analysis of errors, detailed numerical information about results of experiments. A conclusion is made that the available data do not come up to modern requirements. It is necessary to make new measurements of fission prompt neutron spectra of transuranium nuclides important for the objectives of working out a conception of minor actinides transmutation by means of special reactors. (author)
Neutron gamma competition in fast fission
International Nuclear Information System (INIS)
Frehaut, J.
1989-01-01
In the present paper we analyse the data we have obtained on the distribution of the gamma-ray energy per fission, as well as on the average energy E-barγ released per fission for the neutron induced fission of several isotopes, in the energy range up to 15 MeV. 6 refs, 9 figs
A new neutron counter for fission research
Energy Technology Data Exchange (ETDEWEB)
Laurent, B., E-mail: benoit.laurent@cea.fr [CEA, DAM, DIF, F-91297 Arpajon (France); Granier, T.; Bélier, G.; Chatillon, A.; Martin, J.-F.; Taieb, J. [CEA, DAM, DIF, F-91297 Arpajon (France); Hambsch, F.-J. [EC-JRC Institute for Reference Materials and Measurements (IRMM), Retieseweg, 2440 Geel (Belgium); Tovesson, F.; Laptev, A.B.; Haight, R.C.; Nelson, R.O.; O' Donnell, J.M. [Los Alamos Neutron Science Center, Los Alamos National Laboratory, Los Alamos, NM 87545 (United States)
2014-05-01
A new neutron counter for research experiments on nuclear fission has been developed. This instrument is designed for the detection of prompt fission neutrons within relatively high levels of gamma and neutron background. It is composed of a set of {sup 3}He proportional counters arranged within a block of polyethylene which serves as moderator. The detection properties have been studied by means of Monte Carlo simulations and experiments with radioactive sources. These properties are confirmed by an experiment on neutron-induced fission of {sup 238}U at the WNR facility of the Los Alamos Neutron Science Center during which the mean prompt fission neutron multiplicity, or ν{sup ¯} has been measured from 1 to 20 MeV of incident neutron energy.
Neutronics of Laser Fission-Fusion Systems
International Nuclear Information System (INIS)
Velarde, G.
1976-01-01
Neutronics of Fission-Fusion microsystems inertially confined by Lasers are analysed by transport calculation, both stationary (DTF, TIHOC) and time dependent (TDA, TIHEX), discussing the results obtained for the basic parameters of the fission process (multiplication factor, neutron generation time and Rossi-∞). (Author) 14 refs
Neutronics of Laser Fission-Fusion Systems
Energy Technology Data Exchange (ETDEWEB)
Velarde, G
1976-07-01
Neutronics of Fission-Fusion microsystems inertially confined by Lasers are analysed by transport calculation, both stationary (DTF, TIHOC) and time dependent (TDA, TIHEX), discussing the results obtained for the basic parameters of the fission process (multiplication factor, neutron generation time and Rossi-{infinity}). (Author) 14 refs.
Fission and r-process nucleosynthesis in neutron star mergers
International Nuclear Information System (INIS)
Giuliani, Samuel Andrea
2018-01-01
rates are used in r-process calculations for matter dynamically ejected in neutron star mergers and we compare our results with those obtained from a more conventional set of reaction rates. We find that all the models predict the onset of fission above the shell closure N=184 and Z=100 due to the sudden decrease in fission barriers. However, the amount of material accumulated at N=184 turns out to be very sensitive to the height of the fission barriers and the shell gap. Finally, we have also explored the impact of recent advances in fission calculations on the theoretical estimation of spontaneous fission lifetimes. We find that performing dynamical approaches based on the minimization of the integral action with nontraditional collective degrees of freedom has a strong impact in the fission barriers and the spontaneous fission lifetimes. The possible consequences of this new approach for the calculation of neutron induced fission rates has to be addressed.
Measurement of prompt fission gamma-ray spectra in fast neutron-induced fission
International Nuclear Information System (INIS)
Laborie, J.M.; Belier, G.; Taieb, J.
2012-01-01
Knowledge of prompt fission gamma-ray emission has been of major interest in reactor physics for a few years. Since very few experimental spectra were ever published until now, new measurements would be also valuable to improve our understanding of the fission process. An experimental method is currently being developed to measure the prompt fission gamma-ray spectrum from some tens keV up to 10 MeV at least. The mean multiplicity and total energy could be deduced. In this method, the gamma-rays are measured with a bismuth germanate (BGO) detector which has the advantage to present a high P/T ratio and a high efficiency compared to other gamma-ray detectors. The prompt fission neutrons are rejected by the time of flight technique between the BGO detector and a fission trigger given by a fission chamber or a scintillating active target. Energy and efficiency calibration of the BGO detector were carried out up to 10.76 MeV by means of the Al-27(p, gamma) reaction. First prompt fission gamma-ray spectrum measurements performed for the spontaneous fission of Cf-252 and for 1.7 and 15.6 MeV neutron-induced fission of U-238 at the CEA, DAM, DIF Van de Graaff accelerator, will be presented. (authors)
Neutron-induced fission cross sections
International Nuclear Information System (INIS)
Weigmann, H.
1991-01-01
In the history of fission research, neutron-induced fission has always played the most important role. The practical importance of neutron-induced fission rests upon the fact that additional neutrons are produced in the fission process, and thus a chain reaction becomes possible. The practical applications of neutron-induced fission will not be discussed in this chapter, but only the physical properties of one of its characteristics, namely (n,f) cross sections. The most important early summaries on the subject are the monograph edited by Michaudon which also deals with the practical applications, the earlier review article on fission by Michaudon, and the review by Bjornholm and Lynn, in which neutron-induced fission receives major attention. This chapter will attempt to go an intermediate way between the very detailed theoretical treatment in the latter review and the cited monograph which emphasizes the applied aspects and the techniques of fission cross-section measurements. The more recent investigations in the field will be included. Section II will survey the properties of cross sections for neutron-induced fission and also address some special aspects of the experimental methods applied in their measurement. Section Ill will deal with the formal theory of neutron-induced nuclear reactions for the resolved resonance region and the region of statistical nuclear reactions. In Section IV, the fission width, or fission transmission coefficient, will be discussed in detail. Section V will deal with the broader structures due to incompletely damped vibrational resonances, and in particular will address the special case of thorium and neighboring isotopes. Finally, Section VI will briefly discuss parity violation effects in neutron-induced fission. 74 refs., 14 figs., 3 tabs
Dispersions and correlations of the distributions of products of 252Cf spontaneous fission
International Nuclear Information System (INIS)
Vidyakin, G.S.; Vyrodov, V.N.; Gurevich, I.I.; Kirillov, B.F.; Kozlov, Y.V.; Martem'yanov, V.P.; Sukhotin, S.V.; Tarasenkov, V.G.; Khakimov, S.K.
1982-01-01
We report the results of two experiments on study of the dispersions and correlations of the distributions of products of the spontaneous fission of 252 Cf. In each experiment about 10 8 fissions were recorded with simultaneous measurement of the number of neutrons produced and in one case the fragment kinetic energy and in the other case the energy of the prompt #betta# rays. The quantities obtained were the probabilities of production of a given number of neutrons per fission, the dispersions of the distributions of the number of neutrons produced and of the fragment kinetic energy, and the dependence of the average #betta#-ray energy and the average fragment kinetic energy on the number of neutrons produced. A calculation is made of the spectrum of the total energy carried away by fragments and neutrons, and its dispersion is determined. An estimate of the total energy release in the 252 Cf fission process is made
Recent improvements in the calculation of prompt fission neutron spectra: Preliminary results
International Nuclear Information System (INIS)
Madland, D.G.; LaBauve, R.J.; Nix, J.R.
1989-01-01
We consider three topics in the refinement and improvement of our original calculations of prompt fission neutron spectra. These are an improved calculation of the prompt fission neutron spectrum N(E) from the spontaneous fission of 252 Cf, a complete calculation of the prompt fission neutron spectrum matrix N(E,E n ) from the neutron-induced fission of 235 U, at incident neutron energies ranging from 0 to 15 MeV, and an assessment of the scission neutron component of the prompt fission neutron spectrum. Preliminary results will be presented and compared with experimental measurements and an evaluation. A suggestion is made for new integral cross section measurements. (author). 45 refs, 12 figs, 1 tab
Measurement of Fission Product Yields from Fast-Neutron Fission
Arnold, C. W.; Bond, E. M.; Bredeweg, T. A.; Fowler, M. M.; Moody, W. A.; Rusev, G.; Vieira, D. J.; Wilhelmy, J. B.; Becker, J. A.; Henderson, R.; Kenneally, J.; Macri, R.; McNabb, D.; Ryan, C.; Sheets, S.; Stoyer, M. A.; Tonchev, A. P.; Bhatia, C.; Bhike, M.; Fallin, B.; Gooden, M. E.; Howell, C. R.; Kelley, J. H.; Tornow, W.
2014-09-01
One of the aims of the Stockpile Stewardship Program is a reduction of the uncertainties on fission data used for analyzing nuclear test data [1,2]. Fission products such as 147Nd are convenient for determining fission yields because of their relatively high yield per fission (about 2%) and long half-life (10.98 days). A scientific program for measuring fission product yields from 235U,238U and 239Pu targets as a function of bombarding neutron energy (0.1 to 15 MeV) is currently underway using monoenergetic neutron beams produced at the 10 MV Tandem Accelerator at TUNL. Dual-fission chambers are used to determine the rate of fission in targets during activation. Activated targets are counted in highly shielded HPGe detectors over a period of several weeks to identify decaying fission products. To date, data have been collected at neutron bombarding energies 4.6, 9.0, 14.5 and 14.8 MeV. Experimental methods and data reduction techniques are discussed, and some preliminary results are presented.
Attempt to enrich of a new spontaneous fissioning nuclide by evaporation of natural brine
International Nuclear Information System (INIS)
Adamek, A.; Zhuravleva, E.L.; Constantinescu, M.; Constantinescu, o.; Chuburkov, Yu.T.
1983-01-01
The enrichment of the new spontaneous fissioning nuclide discovered in the Cheleken brine, was made by evaporation. The purpose of this work was the comparison of behaviour of the new spontaneous fissioning nuclide with that of the known elements in the formation processes of the high concentration brines. Spontaneous fission of the nuclide was measured by means of the counters for multiple emission of neutrons. It is shown that the new spontaneous fissioning nuclide was enriched as well as other trace elements (Hg, Tl, Bi and Pb) in a solution remained after the evaporation of the initial solution. The conclusion is drawn that from the sea water brines could be obtained by evaporation which are enriched in trace elements with an enrichment degree higher than the natural brines
Nuclear fission and neutron-induced fission cross-sections
James, G D; Michaudon, A; Michaudon, A; Cierjacks, S W; Chrien, R E
2013-01-01
Nuclear Fission and Neutron-Induced Fission Cross-Sections is the first volume in a series on Neutron Physics and Nuclear Data in Science and Technology. This volume serves the purpose of providing a thorough description of the many facets of neutron physics in different fields of nuclear applications. This book also attempts to bridge the communication gap between experts involved in the experimental and theoretical studies of nuclear properties and those involved in the technological applications of nuclear data. This publication will be invaluable to those interested in studying nuclear fis
Theory of neutron emission in fission
International Nuclear Information System (INIS)
Madland, D.G.
1989-01-01
Following a summary of the observables in neutron emission in fission, a brief history is given of theoretical representations of the prompt fission neutron spectrum N(E) and average prompt neutron multiplicity /bar /nu///sub p/. This is followed by descriptions, together with examples, of modern approaches to the calculation of these quantities including recent advancements. Emphasis will be placed upon the predictability and accuracy of the modern approaches. In particular, the dependence of N(E) and /bar /nu///sub p/ on the fissioning nucleus and its excitation energy will be discussed, as will the effects of and competition between first-, second- and third-chance fission in circumstances of high excitation energy. Finally, properties of neutron-rich (fission-fragment) nuclei are discussed that must be better known to calculate N(E) and /bar /nu///sub p/ with higher accuracy than is currently possible. 17 refs., 11 figs
International Nuclear Information System (INIS)
Mikheev, V.L.; Tret'yakova, S.P.; Golovchenko, A.N.; Timofeeva, O.V.; Hussonnois, M.; Le Naour, C.
1998-01-01
The low limit of the 226 Ra spontaneous fission half-life corresponding to T 1/2 ≥ 4 · 10 18 years is measured. The 226 Ra spontaneous fission probability proved to be about 50 times less than the value expected from the known systematics, connecting the ratios of theα-decay and spontaneous fission probabilities with the fissility parameter Z 2 /A. It is shown that the probabilities of spontaneous fission, α-decay and cluster decay can be systematized in the same way according to the difference between the decay products Coulomb energy near the scission point and decay energy Q
Contributions to the theory of fission neutron emission
International Nuclear Information System (INIS)
Seeliger, D.; Maerten, H.; Ruben, A.
1990-03-01
This report gives a compilation of recent work performed at Technical University, Dresden by D. Seeliger, H. Maerten and A. Ruben on the topic of fission neutron emission. In the first paper calculated fission neutron spectra are presented using the temperature distribution model FINESSE for fissioning actinide nuclei. In the second paper, starting from a general energy balance, Terrell's approach is generalized to describe average fragment energies as a function of incident energy; trends of fragment energy data in the Th-Pu region are well reproduced. In the third contribution, prompt fission neutron spectra and fragment characteristics for spontaneous fission of even Pu-isotopes are presented and discussed in comparison with experimental data using a phenomenological scission point model including temperature dependent shell effects. In the fourth paper, neutron multiplicities and energy spectra as well as average fragment energies for incident energies from threshold to 20 MeV (including multiple-chance fission) for U-238 are compared with traditional data representations. (author). Refs, figs and tabs
Dating by fission track method: study of neutron dosimetry with natural uranium thin films
International Nuclear Information System (INIS)
Iunes, P.J.
1990-06-01
Fission track dating is described, focalizing the problem of the decay constant for spontaneous fission of 238 U and the use of neutron dosimetry in fission track analysis. Experimental procedures using thin films of natural uranium as neutron dosimeters and its results are presented. The author shows a intercomparison between different thin films and between the dosimetry with thin film and other dosimetries. (M.V.M.). 52 refs, 12 figs, 9 tabs
The resonance neutron fission on heavy nuclei
International Nuclear Information System (INIS)
Kopach, Yu.N.; Popov, A.B.; Furman, V.I.; Alfimenkov, V.P.; Lason', L.; Pikel'ner, L.B.; ); Gonin, N.N.; Kozlovskij, L.K.; Tambovtsev, D.I.; Gagarskij, A.M.; Petrov, G.A.; Sokolov, V.E.
2001-01-01
A new approach to the description of the fission, similar to the well-known reaction theory and based on the helicity representation for the exit fission channels, is briefly summarized. This approach allows one to connect the multimodal fission representation with A. Bohr's concept of the fission transition states and to obtain formulae for the partial and differential fission cross sections. The formulae are used for analysis of the angular anisotropy of fragments in the neutron resonance induced fission of aligned 235 U nuclei and of the P-even angular forward-backward and right-left correlations of fragments oe the P-odd correlations caused by the interference of s- and p-wave neutron resonances [ru
Mathematical processing of experimental data on neutron yield from separate fission fragments
International Nuclear Information System (INIS)
Basova, B.G.; Rabinovich, A.D.; Ryazanov, D.K.
1975-01-01
The algorithm is described for processing the multi-dimensional experiments on measurements of prompt emission of neutrons from separate fission fragments. While processing the data the effect of a number of experimental corrections is correctly taken into account; random coincidence background, neutron spectrum, neutron detector efficiency, instrument angular resolution. On the basis of the described algorithm a program for BESM-4 computer is realized and the treatment of experimental data is performed according to the spontaneous fission of 252 Cf
International Nuclear Information System (INIS)
Zucker, M.S.; Holden, N.E.
1986-01-01
Recent development in the theory and practice of neutron correlation (''coincidence'') counting require knowledge of the higher factorial moments of the P/sub ν/ distribution (the probability that (ν) neutrons are emitted in a fission) for the case where the fission is induced by bombarding neutrons of more than thermal energies. In contrast to the situation with spontaneous and thermal neutron induced fission, where with a few exceptions the P/sub ν/ is reasonably well known, in the fast neutron energy region, almost no information is available concerning the multiplicity beyond the average value, [ν], even for the most important nuclides. The reason for this is the difficulty of such experiments, with consequent statistically poor and physically inconsistent results
Study of the shielding for spontaneous fission sources of Californium-252
International Nuclear Information System (INIS)
Davila R, I.
1991-06-01
A shielding study is made to attenuate, until maximum permissible levels, the neutrons radiation and photons emitted by spontaneous fission coming from a source of Californium-252. The compound package by a database (Library DLC-23) and the ANISNW code is used, in it version for personal computer. (Author)
Angular distribution of oriented nucleus fission neutrons
International Nuclear Information System (INIS)
Barabanov, A.L.; Grechukhin, D.P.
1982-01-01
Calculations of anisotropy of angular distribution of oriented 235 U nuclei thermal fission neutrons have been carried out. the neutrons were assumed to evaporate isotropically by completely accelerated fragements in the fragment system with only its small part, i. e. fission-producing neutrons, emitted at the moment of neck break. It has been found out that at low energies of neutrons Esub(n)=1-2 MeV the sensitivity of the angular distribution anisotropy to variations of spectrum of neutron evaporation from fragments and the magnitude of a share of fission-producing neutrons reaches approximately 100%, which at high energies, Esub(n) > 5 MeV it does not exceed approximately 20%. Therefore the angular distribution of fast neutrons to a greater degree of confidence may be used for restoring the angular distribution anisotropy of fragments while the angular distribution of low energy neutrons may be used for deriving information on the fission process, but only in case 6f the experiment accuracy is better than approximately 3%
Bhatia, C.; Fallin, B.; Gooden, M. E.; Howell, C. R.; Kelley, J. H.; Tornow, W.; Arnold, C. W.; Bond, E. M.; Bredeweg, T. A.; Fowler, M. M.; Moody, W. A.; Rundberg, R. S.; Rusev, G.; Vieira, D. J.; Wilhelmy, J. B.; Becker, J. A.; Macri, R.; Ryan, C.; Sheets, S. A.; Stoyer, M. A.; Tonchev, A. P.
2014-09-01
A program has been initiated to measure the energy dependence of selected high-yield fission products used in the analysis of nuclear test data. We present out initial work of neutron activation using a dual-fission chamber with quasi-monoenergetic neutrons and gamma-counting method. Quasi-monoenergetic neutrons of energies from 0.5 to 15 MeV using the TUNL 10 MV FM tandem to provide high-precision and self-consistent measurements of fission product yields (FPY). The final FPY results will be coupled with theoretical analysis to provide a more fundamental understanding of the fission process. To accomplish this goal, we have developed and tested a set of dual-fission ionization chambers to provide an accurate determination of the number of fissions occurring in a thick target located in the middle plane of the chamber assembly. Details of the fission chamber and its performance are presented along with neutron beam production and characterization. Also presented are studies on the background issues associated with room-return and off-energy neutron production. We show that the off-energy neutron contribution can be significant, but correctable, while room-return neutron background levels contribute less than <1% to the fission signal.
Theoretical descriptions of neutron emission in fission
International Nuclear Information System (INIS)
Madland, D.G.
1991-01-01
Brief descriptions are given of the observables in neutron emission in fission together with early theoretical representations of two of these observables, namely, the prompt fission neutron spectrum N(E) and the average prompt neutron multiplicity ν-bar p . This is followed by summaries, together with examples, of modern approaches to the calculation of these two quantities. Here, emphasis is placed upon the predictability and accuracy of the new approaches. In particular, the dependencies of N(E) and ν-bar p upon the fissioning nucleus and its excitation energy are discussed. Then, recent work in multiple-chance fission and other recent work involving new measurements are presented and discussed. Following this, some properties of fission fragments are mentioned that must be better known and better understood in order to calculate N(E) and ν-bar p with higher accuracy than is currently possible. In conclusion, some measurements are recommended for the purpose of benchmarking simultaneous calculations of neutron emission and gamma emission in fission. (author). 32 refs, 26 figs
New isomeric states in 152,154,156Nd produced by spontaneous fission of 252Cf
International Nuclear Information System (INIS)
Gautherin, C.; Houry, M.; Korten, W.; Le Coz, Y.; Lucas, R.; Phan, X.H.; Theisen, C.; Belier, G.; Girod, M.; Meot, V.; Peru, S.; Astier, A.; Ducroux, L.; Meyer, M.; Redon, N.
1998-01-01
Isomeric states have been observed in fission-fragments produced by spontaneous fission of 252 Cf. These states are found in neutron rich nuclei of different structure and deformations. About 50 isomeric nuclei have been observed using coincidences between γ-rays identified in EUROGAM II and fission fragments detected in photovoltaic cells (SAPhIR). Lifetimes in the range from 20 ns to 2μs have been measured. Presented calculations based on HFB+D1S force on new measured isomeric states in the 152,154,156 Nd show evidence for K-isomers. (orig.)
Theory of neutron emission in fission
International Nuclear Information System (INIS)
Madland, D.G.
1998-01-01
A survey of theoretical representations of two of the observables in neutron emission in fission is given, namely, the prompt fission neutron spectrum N(E) and the average prompt neutron multiplicity bar ν p . Early representations of the two observables are presented and their deficiencies are discussed. This is followed by summaries and some examples of recent theoretical models for the calculation of these quantities. Emphasis is placed upon the predictability and accuracy of the recent models. In particular, the dependencies of N(E) and bar ν p upon the fissioning nucleus and its excitation energy are treated in detail for the Los Alamos model. Recent work in the calculation of the prompt fission neutron spectrum matrix N(E, E n ), where E n is the energy of the neutron inducing fission, is then discussed. Concluding remarks address the current status of the ability to calculate these observables with confidence, the direction of future theoretical efforts, and limitations to current (and future) approaches. This paper is an extension of a similar paper presented at the International Centre for Theoretical Physics in 1996
Theoretical models of neutron emission in fission
International Nuclear Information System (INIS)
Madland, D.G.
1992-01-01
A brief survey of theoretical representations of two of the observables in neutron emission in fission is given, namely, the prompt fission neutron spectrum N(E) and the average prompt neutron multiplicity bar v p . Early representations of the two observables are presented and their deficiencies are discussed. This is followed by summaries and examples of recent theoretical models for the calculation of these quantities. Emphasis is placed upon the predictability and accuracy of the new models. In particular, the dependencies of N(E) and bar v p upon the fissioning nucleus and its excitation energy are treated. Recent work in the calculation of the prompt fission neutron spectrum matrix N(E,E n ), where E n is the energy of the neutron inducing fission, is then discussed. Concluding remarks address the current status of our ability to calculate these observables with confidence, the direction of future theoretical efforts, and limititations to current and future calculations. Finally, recommendations are presented as to which model should be used currently and which model should be pursued in future efforts
Correlation properties of delayed neutrons from fast neutron induced fission
International Nuclear Information System (INIS)
Piksaikin, V.M.; Isaev, S.G.
1998-01-01
The experimental studies of the energy dependence of the delayed neutron parameters for various fissioning systems has shown that the behavior of a some combination of delayed neutron parameters (group relative abundances a i and half lives T i ) has a similar features. On the basis of this findings the systematics of delayed neutron experimental data for thorium, uranium, plutonium and americium isotopes have been investigated with the purpose to find a correlation of DN parameters with characteristics of fissioning system as well as a correlation between the delayed neutron parameters themselves. Below we will present the preliminary results which were obtained during this study omitting the physics interpretation of the results. (author)
Ternary fission induced by polarized neutrons
Directory of Open Access Journals (Sweden)
Gönnenwein Friedrich
2013-12-01
Full Text Available Ternary fission of (e,e U- and Pu- isotopes induced by cold polarized neutrons discloses some new facets of the process. In the so-called ROT effect shifts in the angular distributions of ternary particles relative to the fission fragments show up. In the so-called TRI effect an asymmetry in the emission of ternary particles relative to a plane formed by the fragment momentum and the spin of the neutron appear. The two effects are shown to be linked to the components of angular momentum perpendicular and parallel to the fission axis at the saddle point of fission. Based on theoretical models the spectroscopic properties of the collective transitional states at the saddle point are inferred from experiment.
Fission neutron spectra measurements at LANSCE - Status and plans
International Nuclear Information System (INIS)
Haight, R. C.; Noda, S.; Nelson, R. O.; O'Donnell, J. M.; Devlin, M.; Chatillon, A.; Granier, T.; Taiebb, J.; Laurent, B.; Belier, G.; Becker, J. A.; Wu, C. Y.
2010-01-01
A program to measure fission neutron spectra from neutron-induced fission of actinides is underway at the Los Alamos Neutron Science Center (LANSCE) in a collaboration among the CEA laboratory at Bruyeres-le-Chatel, Lawrence Livermore National Laboratory and Los Alamos National Laboratory. The spallation source of fast neutrons at LANSCE is used to provide incident neutron energies from less than 1 MeV to 100 MeV or higher. The fission events take place in a gas-ionization fission chamber, and the time of flight from the neutron source to that chamber gives the energy of the incident neutron. Outgoing neutrons are detected by an array of organic liquid scintillator neutron detectors, and their energies are deduced from the time of flight from the fission chamber to the neutron detector. Measurements have been made of the fission neutrons from fission of 235 U, 238 U, 237 Np and 239 Pu. The range of outgoing energies measured so far is from 0.7 MeV to approximately 8 MeV. These partial spectra and average fission neutron energies are compared with evaluated data and with models of fission neutron emission. Results to date are summarized in this presentation. Future plans are to make significant improvements in the fission chambers, neutron detectors, signal processing, data acquisition and the experimental environment to provide high fidelity data including measurements of fission neutrons below 0.7 MeV and improvements in the data above 8 MeV. (authors)
International Nuclear Information System (INIS)
Spaggiari, E.R.V.
1978-01-01
The results of measuments of the disintegration constant for spontaneous fission in 238 U are presented, with a discussion on the method used for the detection of fission tracks in muscovite mica. Samples of muscovite mica sandwiched between two natural uranium dioxide cylinders were irradiated with fragments of spontaneous fission and the etched tracks counted with projetion optical microscope. The effective thickness of the UO 2 layer which contributed to the observed tracks was measured through irradiation of mica samples, in contact with the UO 2 cylinder with 14,0 MeV neutrons from a (d,t) reaction. (Author) [pt
International Nuclear Information System (INIS)
Vasil'ev, Yu.A.; Sidorov, L.V.; Vasil'eva, N.K.; Barashkov, Yu.A.; Golovanov, O.A.; Kopalkin, N.V.; Nemudrov, N.I.; Surin, V.M.; Khachaturov, Yu.F.
1984-01-01
The results of the 4π-spectrometer mesurement of the neutron spectra in the 26-154 deg angle range for seven groups of fragments with different masses and total kinetic energies are given. Experimental spectra have been analyzed for consistency with the evaporation model of neutrons from moving fragments. The results of an analysis of differential neutron spectra shows that the main reason of the ''yearly'' neutron emission is a neutron evaporation from fragments with large excitation energy and from fragments with neutron number N>82 during the time as compared with the time of fragment acceleration
Neutron induced current pulses in fission chambers
International Nuclear Information System (INIS)
Taboas, A.L.; Buck, W.L.
1978-01-01
The mechanism of neutron induced current pulse generation in fission chambers is discussed. By application of the calculated detector transfer function to proposed detector current pulse shapes, and by comparison with actually observed detector output voltage pulses, a credible, semi-empirical, trapezoidal pulse shape of chamber current is obtained
Fission neutron output measurements at LANSCE
International Nuclear Information System (INIS)
Nelson, Ronald Owen; Haight, Robert C.; Devlin, Matthew J.; Fotiadis, Nikolaos; Laptev, Alexander; O'Donnell, John M.; Taddeucci, Terry N.; Tovesson, Fredrik; Ullmann, J.L.; Wender, Stephen A.; Bredeweg, T.A.; Jandel, M.; Vieira, D.J.; Wu, Ching-Yen; Becker, J.A.; Stoyer, M.A.; Henderson, R.; Sutton, M.; Belier, Gilbert; Chatillon, A.; Granier, Thierry; Laurent, Benoit; Taieb, Julien
2010-01-01
Accurate data for both physical properties and fission properties of materials are necessary to properly model dynamic fissioning systems. To address the need for accurate data on fission neutron energy spectra, especially at outgoing neutron energies below about 200 keV and at energies above 8 MeV, ongoing work at LANSCE involving collaborators from LANL, LLNL and CEA Bruyeres-le-Chatel is extending the energy range, efficiency and accuracy beyond previous measurements. Initial work in the outgoing neutron energy range from 1 to 7 MeV is consistent with current evaluations and provides a foundation for extended measurements. As part of these efforts, a new fission fragment detector that reduces backgrounds and improves timing has been designed fabricated and tested, and new neutron detectors are being assessed for optimal characteristics. Simulations of experimental designs are in progress to ensure that accuracy goals are met. Results of these measurements will be incorporated into evaluations and data libraries as they become available.
International Nuclear Information System (INIS)
Zucker, M.S.; Holden, N.E.
1986-01-01
Certain applications require knowledge of the higher moments of the neutron multiplicity probability. It can be shown that the second factorial moment is proportional to the fission rate in the sample, and that the third factorial moment can be of use in disentangling spontaneous fission from induced fission. Using a source of unpublished work in which neutron multiplicities were derived for the fast neutron induced fission of U-235, U-238, and Pu-239, the multiplicity probability has been calculated as a function of neutron energy for the energy range 0 to 10 MeV
Fast-neutron-induced fission of 242Pu at nELBE
Directory of Open Access Journals (Sweden)
Kögler Toni
2017-01-01
Full Text Available The fast neutron-induced fission cross section of 242Pu was determined in the range of 0.5 MeV to 10 MeV relative to 235U(n,f at the neutron time-of-flight facility nELBE. The number of target nuclei was calculated by means of measuring the spontaneous fission rate of 242Pu. Neutron transport simulations with Geant4 and MCNP6 are used to correct the relative cross section for neutron scattering. The determined results are in good agreement with current experimental and evaluated data sets.
International Nuclear Information System (INIS)
Spaggiari, E.R.V.
1980-01-01
Results are presented of measurements realized aiming to determine the disintegration constant of spontaneous fission of U-238, with a discussion of the method utilized in the detection of fission tracks in muscovite. Several blades of mica were placed between two cylinders of Uo 2 to be irradiated with the fragments of spontaneous fission of U-238, and the fission tracks duly enlarged after a convenient chemical action were observed with a projection optical microscope. The effective thickness of UO 2 contributing to the observed tracks was measured through the irradiation of mica samples juxtaposed to the UO 2 cylinder, with 14,0 MeV neutrons from the (d,t 2 ) reaction. The detection efficiency of fission tracks originated in that thickness is practically 100% [pt
Improved fission neutron energy discrimination with {sup 4}He detectors through pulse filtering
Energy Technology Data Exchange (ETDEWEB)
Zhu, Ting, E-mail: ting.zhu@ufl.edu [University of Florida, Gainesville, FL (United States); Liang, Yinong; Rolison, Lucas; Barker, Cathleen; Lewis, Jason; Gokhale, Sasmit [University of Florida, Gainesville, FL (United States); Chandra, Rico [Arktis Radiation Detectors Ltd., Räffelstrasse 11, Zürich (Switzerland); Kiff, Scott [Sandia National Laboratories, CA (United States); Chung, Heejun [Korean Institute for Nuclear Nonproliferation and Control, 1534 Yuseong-daero, Yuseong-gu, Daejeon (Korea, Republic of); Ray, Heather; Baciak, James E.; Enqvist, Andreas; Jordan, Kelly A. [University of Florida, Gainesville, FL (United States)
2017-03-11
This paper presents experimental and computational techniques implemented for {sup 4}He gas scintillation detectors for induced fission neutron detection. Fission neutrons are produced when natural uranium samples are actively interrogated by 2.45 MeV deuterium-deuterium fusion reaction neutrons. Fission neutrons of energies greater than 2.45 MeV can be distinguished by their different scintillation pulse height spectra since {sup 4}He detectors retain incident fast neutron energy information. To enable the preferential detection of fast neutrons up to 10 MeV and suppress low-energy event counts, the detector photomultiplier gain is lowered and trigger threshold is increased. Pile-up and other unreliable events due to the interrogating neutron flux and background radiation are filtered out prior to the evaluation of pulse height spectra. With these problem-specific calibrations and data processing, the {sup 4}He detector's accuracy at discriminating fission neutrons up to 10 MeV is improved and verified with {sup 252}Cf spontaneous fission neutrons. Given the {sup 4}He detector's ability to differentiate fast neutron sources, this proof-of-concept active-interrogation measurement demonstrates the potential of special nuclear materials detection using a {sup 4}He fast neutron detection system.
Systematics of neutron-induced fission yields
International Nuclear Information System (INIS)
Blachot, J.; Brissot, R.
1983-10-01
The main characteristics of the mass and charge distributions for thermal neutron induced fission of actinides are reviewed. We show that these distributions can be reasonably reproduced with only 24 data as input. We use a representation where the element yields together with the most probable mass Ap(Z) play the dominant role. The ability of this model to calculate mass yields for the fission of not yet measured actinides is also shown. The influence of the excitation energy of the fissile system on charge and mass distribution is also discussed
Pulsed neutron uranium borehole logging with prompt fission neutrons
International Nuclear Information System (INIS)
Bivens, H.M.; Smith, G.W.; Jensen, D.H.
1976-01-01
The gross count natural gamma log normally used for uranium borehole logging is seriously affected by disequilibrium. Methods for the direct measurement of uranium, such as neutron logging, which are not affected by disequilibrium have been the object of considerable effort in recent years. This paper describes a logging system for uranium which uses a small accelerator to generate pulses of 14 MeV neutrons to detect and assay uranium by the measurement of prompt fission neutrons in the epithermal energy range. After an initial feasibility study, a prototype logging probe was built for field evaluation which began in January 1976. Physical and operational characteristics of the prototype probe, the neutron tube-transformer assembly, and the neutron tube are described. In logging operations, only the epithermal prompt fission neutrons detected between 250 microseconds to 2500 microseconds following the excitation neutron pulse are counted. Comparison of corrected neutron logs with the conventional gross count natural gamma logs and the chemical assays of cores from boreholes are shown. The results obtained with this neutron probe clearly demonstrate its advantages over the gross count natural gamma log, although at this time the accuracy of the neutron log assay is not satisfactory under some conditions. The necessary correction factors for various borehole and formation parameters are being determined and, when applied, should improve the assay accuracy
Study of ternary and quaternary spontaneous fission of 252Cf with the NESSI detector
International Nuclear Information System (INIS)
Tishchenko, V.G.; Jahnke, U.; Herbach, C.M.; Hilscher, D.
2002-11-01
Ternary and quaternary spontaneous decay of 252 Cf was studied with the NESSI detector, a combination of two 4π detectors for charged particles, neutrons and γ-rays. The applied method of particle identification by measuring the energies and relative time-of-flights of the decay products is shown to be very effective for the study of rare decay modes. The energy and angular distributions of the decay products, the associated neutron multiplicities, the total energy of the prompt γ-radiation as well as correlations between the various observables were measured for the first time in a single full-scale experiment. The characteristics of ternary fission known from previous investigations are confirmed in the frame of a methodically independent experiment. Preliminary estimates of the quaternary fission yield are presented. An attempt is made to determine the mechanism of quaternary fission. (orig.)
A standard fission neutron irradiation facility
International Nuclear Information System (INIS)
Sahasrabudhe, S.G.; Chakraborty, P.P.; Iyer, M.R.; Kirthi, K.N.; Soman, S.D.
1979-01-01
A fission neutron irradiation facility (FISNIF) has been set up at the thermal column of the CIRUS reactor at BARC. The spectrum and the flux have been measured using threshold detectors. The paper describes the setting up of the facility, measurement and application. A concentric cylinder containing UO 2 powder sealed inside surrounds the irradiation point of a pneumatic sample transfer system located in the thermal column of the reactor. Samples are loaded in a standard aluminium capsule with cadmium lining and transported pneumatically. A sample transfer time of 1 s can be achieved in the facility. Typical applications of the facility for studying activation of iron and sodium in fission neutrons are also discussed. (Auth.)
Verbeke, Jérôme M.; Petit, Odile; Chebboubi, Abdelhazize; Litaize, Olivier
2018-01-01
Fission modeling in general-purpose Monte Carlo transport codes often relies on average nuclear data provided by international evaluation libraries. As such, only average fission multiplicities are available and correlations between fission neutrons and photons are missing. Whereas uncorrelated fission physics is usually sufficient for standard reactor core and radiation shielding calculations, correlated fission secondaries are required for specialized nuclear instrumentation and detector modeling. For coincidence counting detector optimization for instance, precise simulation of fission neutrons and photons that remain correlated in time from birth to detection is essential. New developments were recently integrated into the Monte Carlo transport code TRIPOLI-4 to model fission physics more precisely, the purpose being to access event-by-event fission events from two different fission models: FREYA and FIFRELIN. TRIPOLI-4 simulations can now be performed, either by connecting via an API to the LLNL fission library including FREYA, or by reading external fission event data files produced by FIFRELIN beforehand. These new capabilities enable us to easily compare results from Monte Carlo transport calculations using the two fission models in a nuclear instrumentation application. In the first part of this paper, broad underlying principles of the two fission models are recalled. We then present experimental measurements of neutron angular correlations for 252Cf(sf) and 240Pu(sf). The correlations were measured for several neutron kinetic energy thresholds. In the latter part of the paper, simulation results are compared to experimental data. Spontaneous fissions in 252Cf and 240Pu are modeled by FREYA or FIFRELIN. Emitted neutrons and photons are subsequently transported to an array of scintillators by TRIPOLI-4 in analog mode to preserve their correlations. Angular correlations between fission neutrons obtained independently from these TRIPOLI-4 simulations, using
Prompt fission neutron spectra of n + 235U above the (n, nf) fission threshold
International Nuclear Information System (INIS)
Shu Nengchuan; Chen Yongjing; Liu Tingjin; Jia Min
2015-01-01
Calculations of prompt fission neutron spectra (PFNS) from the 235 U(n, f) reaction were performed with a semi-empirical method for En = 7.0 and 14.7 MeV neutron energies. The total PFNS were obtained as a superposition of (n, xnf) pre-fission neutron spectra and post-fission spectra of neutrons which were evaporated from fission fragments, and these two kinds of spectra were taken as an expression of the evaporation spectrum. The contributions of (n, xnf) fission neutron spectra on the calculated PFNS were discussed. The results show that emission of one or two neutrons in the (n, nf) or (n, 2nf) reactions influences the PFNS shape, and the neutron spectra of the (n, xnf) fission-channel are soft compared with the neutron spectra of the (n, f) fission channel. In addition, analysis of the multiple-chance fission component showed that second-chance fission dominates the PFNS with an incident neutron energy of 14.7 MeV whereas first-chance fission dominates the 7 MeV case. (authors)
Fission neutron spectra measurements at LANSCE - status and plans
International Nuclear Information System (INIS)
Haight, Robert C.; Noda, Shusaku; Nelson, Ronald O.; O' Donnell, John M.; Devlin, Matt; Chatillon, Audrey; Granier, Thierry; Taieb, Julien; Laurent, Benoit; Belier, Gilbert; Becker, John A.; Wu, Ching-Yen
2009-01-01
A program to measure fission neutron spectra from neutron-induced fission of actinides is underway at the Los Alamos Neutron Science Center (LANSCE) in a collaboration among the CEA laboratory at Bruyeres-le-Chatel, Lawrence Livermore National Laboratory and Los Alamos National Laboratory. The spallation source of fast neutrons at LANSCE is used to provide incident neutron energies from less than 1 MeV to 100 MeV or higher. The fission events take place in a gas-ionization fission chamber, and the time of flight from the neutron source to that chamber gives the energy of the incident neutron. Outgoing neutrons are detected by an array of organic liquid scintillator neutron detectors, and their energies are deduced from the time of flight from the fission chamber to the neutron detector. Measurements have been made of the fission neutrons from fission of 235 U, 238 U, 237 Np and 239 Pu. The range of outgoing energies measured so far is from 1 MeV to approximately 8 MeV. These partial spectra and average fission neutron energies are compared with evaluated data and with models of fission neutron emission. Results to date will be presented and a discussion of uncertainties will be given in this presentation. Future plans are to make significant improvements in the fission chambers, neutron detectors, signal processing, data acquisition and the experimental environment to provide high fidelity data including mea urements of fission neutrons below 1 MeV and improvements in the data above 8 MeV.
Asymmetry of mass and charge division in spontaneous fission
International Nuclear Information System (INIS)
Chakraborty, P.P.; Iyer, M.R.; Ganguly, A.K.
The order-disorder model (ODM) has been used to explain asymmetry of mass and charge division and related phenomena in fission. According to this model the fission process involves two steps consisting of charge polarisation into two impending fragments with beta stable neutron numbers and subsequent distribution of the balance neutrons between the two. The statistics developed on the principle of equal a priori probability of all charge polarisation is used. The shell effects comes into play only in deciding stable neutron number for the charges. The total isotopic yield distribution for a number of fission reactions are presented. These show asymmetry in the actinide region which reduces with increasing mass/charge of the fissioning nuclide and bunching of the higher z peaks. The mass yields obtained therefrom for a number of fission reactions are compared with experimental results. Though there is general agreement with experimental data, the peaks of the distributions are slightly shifted away from the symmetric point and the distributions are somewhat narrower. Charge distribution parameters obtained from these results are also presented. The model predicts preference of asymmetric division for super heavy nuclides. (author)
Determination of the fast-neutron-induced fission cross-section of 242Pu at nELBE
Kögler, Toni; Beyer, Roland; Junghans, Arnd R.; Schwengner, Ronald; Wagner, Andreas
2018-03-01
The fast-neutron-induced fission cross section of 242Pu was determined in the energy range of 0.5 MeV to 10MeV at the neutron time-of-flight facility nELBE. Using a parallel-plate fission ionization chamber this quantity was measured relative to 235U(n,f). The number of target nuclei was thereby calculated by means of measuring the spontaneous fission rate of 242Pu. An MCNP 6 neutron transport simulation was used to correct the relative cross section for neutron scattering. The determined results are in good agreement with current experimental and evaluated data sets.
Determination of the fast-neutron-induced fission cross-section of 242Pu at nELBE
Directory of Open Access Journals (Sweden)
Kögler Toni
2018-01-01
Full Text Available The fast-neutron-induced fission cross section of 242Pu was determined in the energy range of 0.5 MeV to 10MeV at the neutron time-of-flight facility nELBE. Using a parallel-plate fission ionization chamber this quantity was measured relative to 235U(n,f. The number of target nuclei was thereby calculated by means of measuring the spontaneous fission rate of 242Pu. An MCNP 6 neutron transport simulation was used to correct the relative cross section for neutron scattering. The determined results are in good agreement with current experimental and evaluated data sets.
{sup 235}U(n,F) prompt fission neutron spectra
Energy Technology Data Exchange (ETDEWEB)
Maslov, M.V.; Tetereva, N.A. [Joint Institute of Nuclear and Energy Research, Minsk-Sosny (Belarus); Pronyaev, V.P.; Kagalenko, A.B. [Institute of Physics and Power Engineering, Obninsk (Russian Federation); Capote, R. [International Atomic Energy Agency, Vienna (Austria); Granier, T.; Morillon, B. [CEA, Centre DAM-IIe de France, 91 - Arpajon (France); Hambsch, F.J. [EC-JRC Institute for Reference Materials and Measurements, Geel (Belgium); Sublet, J.C. [CEA Cadarache, 13 - Saint Paul lez Durance (France)
2009-07-01
The longstanding problem of inconsistency of integral thermal data testing and differential prompt fission neutron spectra data (PFNS) is mostly due to rather poor fits of differential PFNS data in major data libraries. The measured database is updated by using modern standards including Manhart's evaluation of the spontaneous fission neutron spectra of {sup 252}Cf(sf). That largely removes the inconsistency of older thermal neutron-induced PFNS measurements with newest data of JRC IRMM by Hambsch et al. (2009). A phenomenological approach, developed by Kornilov et al. (1999), for the first-chance fission and extended for the emissive fission domain by Maslov et al. (2005) is calibrated at E{sub th} to predict both the PFNS average energy
Improved Fission Neutron Data Base for Active Interrogation of Actinides
Energy Technology Data Exchange (ETDEWEB)
Pozzi, Sara; Czirr, J. Bart; Haight, Robert; Kovash, Michael; Tsvetkov, Pavel
2013-11-06
This project will develop an innovative neutron detection system for active interrogation measurements. Many active interrogation methods to detect fissionable material are based on the detection of neutrons from fission induced by fast neutrons or high-energy gamma rays. The energy spectrum of the fission neutrons provides data to identify the fissionable isotopes and materials such as shielding between the fissionable material and the detector. The proposed path for the project is as follows. First, the team will develop new neutron detection systems and algorithms by Monte Carlo simulations and bench-top experiments. Next, They will characterize and calibrate detection systems both with monoenergetic and white neutron sources. Finally, high-fidelity measurements of neutron emission from fissions induced by fast neutrons will be performed. Several existing fission chambers containing U-235, Pu-239, U-238, or Th-232 will be used to measure the neutron-induced fission neutron emission spectra. The challenge for making confident measurements is the detection of neutrons in the energy ranges of 0.01 – 1 MeV and above 8 MeV, regions where the basic data on the neutron energy spectrum emitted from fission is least well known. In addition, improvements in the specificity of neutron detectors are required throughout the complete energy range: they must be able to clearly distinguish neutrons from other radiations, in particular gamma rays and cosmic rays. The team believes that all of these challenges can be addressed successfully with emerging technologies under development by this collaboration. In particular, the collaboration will address the area of fission neutron emission spectra for isotopes of interest in the advanced fuel cycle initiative (AFCI).
International Nuclear Information System (INIS)
Brunson, G.S. Jr.
1982-06-01
An array of eight high-speed plastic scintillation detectors has been used to infer a mathematical model for the emission multipliciy of prompt gammas in the spontaneous fission of 252 Cf. Exceptional time resolution and coincidence capability permitted the separation of gammas from fast neutrons over a flight path of approximately 10 cm. About 20 different distribution models were tested. The average energy of the prompt gammas is inversely related to the number emitted; however, this inverse relationship is not strong and the total gamma energy does increase with increasing gamma number. An extension of the experiment incorporated a lithium-drifted germanium gamma spectrometer that resolved nearly 100 discrete gammas associated with fission. Of these gammas, some were preferentially associated with fission in which few gammas were emitted. Certain others were more frequent when many gammas were emitted. Results are presented
Evaluation of mass distribution data from 252Cf spontaneous fission
International Nuclear Information System (INIS)
Liu Tingjin
2003-01-01
The mass distribution data of 252 Cf spontaneous fission were evaluated based on 7 sets of available experimental data. The measured data were corrected for the standards and γ intensity used by using the new evaluated ones. The errors were made necessary adjusting. The evaluated experimental data were fitted with spline function without any restriction and with symmetric restriction. These two sets of fit data were recommended as reference data of the mass distribution of 252 Cf spontaneous fission. The errors of the recommended data were considerably reduced comparing with the measured ones. The light and heavy peaks are not completely symmetric. Also there are fine structures on the right side of the light peak at A=109-111 and left side of the heavy peak at A=137-139. These should be paid attention and studied further. (author)
Determination of the neutron-induced fission cross section of 242Pu
International Nuclear Information System (INIS)
Koegler, Toni Joerg
2016-01-01
Neutron induced fission cross sections of actinides like the Pu-isotopes are of relevance for the development of nuclear transmutation technologies. For 242 Pu, current uncertainties are of around 21%. Sensitivity studies show that the total uncertainty has to be reduced to below 5% to allow for reliable neutron physics simulations. This challenging task was performed at the neutron time-of-flight facility of the new German National Center for High Power Radiation Sources at HZDR, Dresden. Within the TRAKULA project, thin, large and homogeneous deposits of 235 U and 242 Pu have been produced successfully. Using two consecutively placed fission chambers allowed the determination of the neutron induced fission cross section of 242 Pu relative to 235 U. The areal density of the Plutonium targets was calculated using the measured spontaneous fission rate. Experimental results of the fast neutron induced fission of 242 Pu acquired at nELBE will be presented and compared to recent experiments and evaluated data. Corrections addressing the neutron scattering are discussed by using results of different neutron transport simulations (Geant 4, MCNP 6 and FLUKA).
New isomeric states in {sup 152,154,156}Nd produced by spontaneous fission of {sup 252}Cf
Energy Technology Data Exchange (ETDEWEB)
Gautherin, C.; Houry, M.; Korten, W.; Le Coz, Y.; Lucas, R.; Phan, X.H.; Theisen, C. [Commissariat l`Energie Atomique de Saclay, Gif sur Yvette (France). DSM/DAPINA/SPhN; Badimon, C.; Barreau, G.; Doan, T.P.; Pedemay, G. [Centre d`Etudes Nucleaires de Bordeaux-Gradignan, Domaine du Haut Vigneau, F-33175 Gradignan (France); Belier, G.; Girod, M.; Meot, V.; Peru, S. [Commissariat a l`Energie Atomique de Bruyeres-le-Chatel, DAM/SPN, BP12, F-91680 Bruyeres-le-Chatel (France); Astier, A.; Ducroux, L.; Meyer, M.; Redon, N. [Institut de Physique Nucleaire de Lyon, F-69622 Villeurbanne Cedex (France)
1998-04-01
Isomeric states have been observed in fission-fragments produced by spontaneous fission of {sup 252}Cf. These states are found in neutron rich nuclei of different structure and deformations. About 50 isomeric nuclei have been observed using coincidences between {gamma}-rays identified in EUROGAM II and fission fragments detected in photovoltaic cells (SAPhIR). Lifetimes in the range from 20 ns to 2{mu}s have been measured. Presented calculations based on HFB+D1S force on new measured isomeric states in the {sup 152,154,156}Nd show evidence for K-isomers. (orig.) With 8 figs., 27 refs.
238U subthreshold neutron induced fission cross section
International Nuclear Information System (INIS)
Difilippo, F.C.; Perez, R.B.; De Saussure, G.; Olsen, D.K.; Ingle, R.W.
1976-01-01
High resolution measurements of the 238 U neutron induced fission cross section are reported for neutron energies between 600 eV and 2 MeV. The average subthreshold fission cross section between 10 and 100 keV was found to be 44 +- 6 μb
Prompt neutrons from {sup 236}U fission fragments
Energy Technology Data Exchange (ETDEWEB)
Boldeman, J W; Musgrove, A.R. de L.; Walsch, R L
1971-03-01
Measurements were made of prompt neutron emission in the thermal neutron fission of {sup 235}U. The mean neutron emission per fragment was obtained for particular values of the fragment mass and total kinetic energy. A direct neutron counting method was employed and a comparison made with data from previous experiments of this type. (author)
An absolute measurement of 252Cf prompt fission neutron spectrum at low energy range
International Nuclear Information System (INIS)
Lajtai, A.; Dyachenko, P.P.; Kutzaeva, L.S.; Kononov, V.N.; Androsenko, P.A.; Androsenko, A.A.
1983-01-01
Prompt neutron energy spectrum at low energies (25 keV 252 Cf spontaneous fission has been measured with a time-of-flight technique on a 30 cm flight-path. Ionization chamber and lithium-glass were used as fission fragment and neutron detectors, respectively. Lithium glasses of NE-912 (containing 6 Li) and of NE-913 (containing 7 Li) 45 mm in diameter and 9.5 mm in thickness have been employed alternatively, for the registration of fission neutrons and gammas. For the correct determination of the multiscattering effects - the main difficulty of the low energy neutron spectrum measurements - a special geometry for the neutron detector was used. Special attention was paid also to the determination of the absolute efficiency of the neutron detector. The real response function of the spectrometer was determined by a Monte-Carlo calculation. The scattering material content of the ionization chamber containing a 252 Cf source was minimized. As a result of this measurement a prompt fission neutron spectrum of Maxwell type with a T=1.42 MeV parameter was obtained at this low energy range. We did not find any neutron excess or irregularities over the Maxwellian. (author)
International Nuclear Information System (INIS)
Vasil'ev, Yu.A.; Barashkov, Yu.A.; Golovanov, O.A.; Sidorov, L.V.
1977-01-01
A method for determining the average number of secondary neutrons anti ν produced in nuclear fission by the neutrons of the 252 Cf fission spectra by means of a 4π time-of-flight spectrometer is described. Layers of 252 Cf and an isotope studied are placed close to each other; if the isotope layer density is 1 mg/cm 2 probability of its fission is about 10 -5 per one spontaneous fission of californium. Fission fragments of 252 Cf and the isotope investigated have been detected by two surface-barrier counters with an efficiency close to 100%. The layers and the counters are situated in a measuring chamber placed in the center of the 4π time-of-flight spectrometer. The latter is utilized as a neutron counter because of its fast response. The method has been verified by carrying out measurements for 235 U and 239 Pu. A comparison of the experimental and calculated results shows that the method suggested can apply to determine the number of secondary neutrons in fission of isotopes that have not been investigated yet
A spike of 4298Mo in yields of uranium spontaneous fission an extension of shell structure effect
International Nuclear Information System (INIS)
Masuda, Akimasa; Takahashi, Kazuya; Kawashima, Atsumichi.
1993-01-01
The investigations of the isotopic abundance ratios of molybdenum in zircon have shown that the molybdenum isotopic composition obtained reflects two effects: (1) spontaneous fission of 92 238 U contained in the zircon and (2) double beta decay of 40 96 Zr. Interestingly, however, the products due to the spontaneous fission appear to have a strange large excess (spike) of 42 98 Mo. It intrigues us that 92 minus 42 leaves 50, one of the outstanding magic numbers. It is suggested in the present communication that the strange spike of 42 98 Mo in question can result from a special type of spontaneous fission having essential bearings on the magic number 50 of protons and the 'magical' numbers 58 and 92 of neutrons. (author)
Correlated spins of complementary fragment pairs in the spontaneous fission of 252Cf
International Nuclear Information System (INIS)
Smith, A. G.; Simpson, G. S.; Billowes, J.; Dagnall, P. J.; Durell, J. L.; Freeman, S. J.; Leddy, M.; Phillips, W. R.; Roach, A. A.; Smith, J. F.
1999-01-01
A study of the γ-ray decay of low-lying excited states in fragments produced in the spontaneous fission of 252 Cf has revealed a significant correlation between the angles of emission of the 2 1 + →0 1 + transitions of complementary fragment pairs. Calculations of the amount of dealignment that is needed to reproduce the measured a 2 values, and a comparison with the results of previous fragment-γ angular distribution measurements, suggests that at scission there may be significant population of m≠0 substates associated with the projection of the fragment spin vector on the fission axis. Fragments from the spontaneous fission of 248 Cm emit 2 1 + →0 1 + γ rays that show markedly reduced interfragment correlations, suggesting that either a larger role is played by the relative angular momentum of the fragments, or that the dealignment introduced by the neutron emission and statistical γ decay to the 2 1 + state is larger in 248 Cm than 252 Cf fission. (c) 1999 The American Physical Society
Simultaneous investigation of fission fragments and neutrons in 252Cf(s,f)
International Nuclear Information System (INIS)
Budtz-Joergensen, C.; Knitter, H.H.
1986-01-01
The gridded twin ion chamber developed at CBNM is used to measure the kinetic energy-, mass- and angular distributions of the fission fragments of 252 Cf in an advantageous 4π-geometry. Together with a neutron time-of-flight detector this experimental arrangement permits to measure the correlation between neutron emission, fragment angle, mass and energy in the spontaneous fission of 252 Cf. With the present experimental set-up a mass resolution for fission fragments of 0.5 a.m.u., an angular resolution of Δcosθ = 0.05 and a timing resolution of 0.7 ns FWHM were observed. Preliminary evaluations of the raw experimental data are presented for the fission fragment mass distribution, the average total kinetic energy and their variance as function of mass, the angular distribution between fragments and neutrons, the number of neutrons emitted per fragment as function of fragment mass, the average neutron emission energies as function of mass, and the prompt fission neutron spectrum averaged over all fragments. (author)
Measurement of the neutron-induced fission cross-section of 240,242Pu
International Nuclear Information System (INIS)
Salvador-Castineira, P.; Hambsch, F.J.; Brys, T.; Oberstedt, S.; Vidali, M.; Pretel, C.
2014-01-01
Fast spectrum neutron-induced fission cross-section data for transuranic isotopes are in high demand in the nuclear data community. In particular, highly accurate data are needed for the new Generation-IV nuclear applications. The aim is to obtain precise neutron-induced fission cross-sections for 240 Pu and 242 Pu. In this context accurate data on spontaneous fission half-lives have also been measured. To minimise the total uncertainty on the fission cross-sections the detector efficiency has been studied in detail. Both isotopes have been measured using a twin Frisch-grid ionisation chamber (TFGIC) due to its superiority compared to other detector systems in view of radiation hardness, 2 x 2π solid angle coverage and very good energy resolution. (authors)
A method for prediction of prompt fission neutron spectra
International Nuclear Information System (INIS)
Grashin, A.F.; Lepeshkin, M.V.
1988-01-01
Three-parameter formula for the prompt-fission-neutron integral spectrum is derived from a thermodynamical model. Two parameters, scission-neutron weight p = 11 % and anisotropy factor for accelerated fragments b = 10 %, are determined from experimental data, the same values being assumed for any type of fission. The thermodynamical theory provides the value of the third parameter, temperature τ, thus prognozing neutron spectrum and average energy with an error about 1 %. (author)
Independent fission yields of Rb and Cs from thermal-neutron-induced fission of 239Pu
International Nuclear Information System (INIS)
Balestrini, S.J.; Forman, L.
1975-01-01
The relative independent fission yields of Rb and Cs from thermal-neutron-induced fission of 239 Pu have been measured on line using a mass spectrograph and thermalized neutrons from a burst reactor. Independent yields were derived by normalizing the measurements to products of chain yields and fractional independent yields, estimating the latter from measured cumulative yields of Kr and Xe. Comparing the independent yields with those from 238 U fission, the 239 Pu results show shifts in isotopic yield distribution toward lower mass for both Rb and Cs and also toward the production of more Cs and less Rb when 239 Pu is fissioned
Dynamic of fission and quasi-fission revealed by pre-scission neutron evaporation
International Nuclear Information System (INIS)
Hinde, D.J.
1991-06-01
The dependence of pre-scission neutron multiplicities (ν-pre) on the mass-split and total kinetic energy (TKE) in fusion-fission and quasi-fission has been measured for a wide range of projectile-target combinations. the data indicate that the fusion-fission time scale is shorter for asymmetric splits than for symmetric splits, whilst there is no dependence on TKE. For quasi-fission reactions induced using 64 Ni projectiles, ν-pre falls rapidly with increasing TKE, indicating that these neutrons are emitted near to or after scission. A new interpretation of both neutron multiplicities and mean energies (the neutron clock-thermometer) allows the extraction of time scales with much less uncertainty than previously, and also gives information about the deformation from which the neutrons are emitted. 15 refs., 13 figs
Energy Technology Data Exchange (ETDEWEB)
Jacob, M [Commissariat a l' Energie Atomique, Saclay (France). Centre d' Etudes Nucleaires
1958-07-01
Study of the number of neutrons produced by fission of {sup 239}Pu. The counting by coincidence of fissions and neutrons produced by these fissions allows the study of the variation of the mean number of neutrons emitted by {nu} fission. In the first chapter, it studied the variation of the mean number of neutrons emitted by {sup 239}Pu fission with the energy of the incident neutron. A description of the experiment is given: a spectrometer with a crystal of sodium chloride or beryllium (mounted on a goniometer) is used, a fission chamber containing 10 mg of {sup 239}Pu and the neutron detection system constituted of BF{sub 3} counters which are enriched in {sup 10}B. In the second part, the counting by coincidence of fissions and neutrons produced by the same fission and received by two different groups of counters allow the determination of a relationship between the root mean square and the average of neutron number produced by fission. The variation of the mean number of neutrons emitted by fission of {sup 239}Pu is studied when we change from a thermal spectra of neutrons to a fission spectra of incident neutrons. Finally, when separating in two different part the fission chamber, it is possible to measure the mean number of neutrons emitted from fission of two different sources. It compared the mean number of neutrons emitted by fission of {sup 239}Pu and {sup 233}U. (M.P.)
Actinide neutron-induced fission cross section measurements at LANSCE
Energy Technology Data Exchange (ETDEWEB)
Tovesson, Fredrik K [Los Alamos National Laboratory; Laptev, Alexander B [Los Alamos National Laboratory; Hill, Tony S [INL
2010-01-01
Fission cross sections of a range of actinides have been measured at the Los Alamos Neutron Science Center (LANSCE) in support of nuclear energy applications in a wide energy range from sub-thermal energies up to 200 MeV. A parallel-plate ionization chamber are used to measure fission cross sections ratios relative to the {sup 235}U standard while incident neutron energies are determined using the time-of-flight method. Recent measurements include the {sup 233,238}U, {sup 239-242}Pu and {sup 243}Am neutron-induced fission cross sections. Obtained data are presented in comparison with ex isting evaluations and previous data.
Survey of neutron spectra generated by the fission of heavy nuclei induced by fast neutrons
International Nuclear Information System (INIS)
Lovchikova, G.N.; Trufanov, A.M.
1997-01-01
A review of neutron fission spectra measurements is presented. This review and the results of this analysis was performed with the participation of the authors. It is shown that there is a need for additional measurements of the energy and angular distributions of secondary neutrons in order to improve the understanding of the neutron emission mechanism in fission. (author). 21 refs, 6 figs
Simultaneous measurement of neutrons and fission fragments of thermal neutron fission of U-233
International Nuclear Information System (INIS)
Itsuro Kimura; Katsuhisa Nishio; Yoshihiro Nakagome
2000-01-01
The multiplicity and the energy of prompt neutrons from the fragments for 233 U(n th , f) were measured as functions of fragment mass and total kinetic energy. Average neutron energy against the fragment mass showed a nearly symmetric distribution about the half mass division with two valleys at 98 and 145 u. The slope of the neutron multiplicity with total kinetic energy depended on the fragment mass and showed the minimum at about 130 u. The obtained neutron data were applied to determine the total excitation energy of the system, and the resulting value in the typical asymmetric fission lied between 22 and 25 MeV. The excitation energy agreed with that determined by subtracting the total kinetic energy from the Q-value within 1 MeV, thus satisfied the energy conservation. In the symmetric fission, where the mass yield was drastically suppresses, the total excitation energy is significantly large and reaches to about 40 MeV, suggesting that fragment pairs are preferentially formed in a compact configuration at the scission point [ru
Prompt neutron emission; Emission des neutrons prompts de fission
Energy Technology Data Exchange (ETDEWEB)
Sher, R [Commissariat a l' Energie Atomique, Saclay (France).Centre d' Etudes Nucleaires
1959-07-01
It is shown that Ramanna and Rao's tentative conclusion that prompt fission neutrons are emitted (in the fragment system) preferentially in the direction of fragment motion is not necessitated by their angular distribution measurements, which are well explained by the usual assumptions of isotropic emission with a Maxwell (or Maxwell-like) emission spectrum. The energy distribution (Watt spectrum) and the angular distribution, both including the effects of anisotropic emission, are given. (author) [French] On montre que la conclusion experimentale de Ramanna et Rao selon laquelle les neutrons prompts de fission sont emis (dans le systeme de reference des fragments) preferentiellement dans la direction du mouvement du fragment, ne decoule pas necessairement de leurs mesures de distribution angulaire. Celles-ci sont bien expliquees par l'hypothese classique de l'emission isotrope et d'un spectre d'emission maxwellien (ou quasi-maxwellien). On donne la distribution en energie (ou spectre de Watt) et la distribution angulaire, comprenant toutes les deux les effets d'emission anisotrope. (auteur)
Delayed neutron yield from fast neutron induced fission of 238U
International Nuclear Information System (INIS)
Piksaikin, V.M.; Kazakov, L.E.; Isaev, S.G.; Roshchenko, V.A.; Goverdovski, A.A.; Tertytchnyi, R.G.
2002-01-01
The measurements of the total delayed neutron yield from fast neutron induced fission of 238 U were made. The experimental method based on the periodic irradiation of the fissionable sample by neutrons from a suitable nuclear reaction had been employed. The preliminary results on the energy dependence of the total delayed neutron yield from fission of 238 U are obtained. According to the comparison of experimental data with our prediction based on correlation properties of delayed neutron characteristics, it is concluded that the value of the total delayed neutron yield near the threshold of (n,f) reaction is not a constant. (author)
Belozerov, A V; Chepigin, V I; Drobina, T P; Gorshkov, V A; Kabachenko, A P; Malyshev, O N; Merkin, I M; Oganessian, Yu T; Popeko, A G; Sagaidak, R N; Svirikhin, A I; Yeremin, A V; Berek, G; Brida, I; Sáro, S
2003-01-01
Heavy-ion fusion reactions sup 4 sup 8 Ca+ sup 2 sup 0 sup 4 Pb and sup 4 sup 4 Ca+ sup 2 sup 0 sup 8 Pb leading to the same compound nucleus sup 2 sup 5 sup 2 No sup * were run in attempts to produce new neutron-deficient spontaneous-fission isotopes of sup 2 sup 4 sup 9 sup , sup 2 sup 5 sup 0 No using the electrostatic separator VASSILISSA. Production cross-sections for the spontaneous-fission activities with the half-lives 5.6 and 54 mu s observed in these reactions are compared with the measured ones for the well-known isotopes of sup 2 sup 5 sup 1 sup - sup 2 sup 5 sup 5 No formed in the heavy-ion fusion reactions sup 4 sup 8 Ca+ sup 2 sup 0 sup 6 Pb and sup 4 sup 8 Ca+ sup 2 sup 0 sup 8 Pb. The obtained excitation functions for the reaction products formed after the evaporation of 1-4 neutrons from the corresponding compound No nuclei have been compared with similar data obtained earlier and results of statistical model calculations. (orig.)
The study of prompt neutron spectra of 238U fission induced by fast neutron
International Nuclear Information System (INIS)
Li Anli; Bai Xixiang; Wang Yufeng; Wang Xiaozhong; Men Jiangchen; Huang Shengnian
1990-01-01
The measurements of prompt neutron time-of-flight spectra of U fission induced by 11 MeV neutrons were carried out at HI-13 Tandem Van de Graaff Accelerator Laboratory in 1989. The block diagram of the electronics is shown. A fission neutron TOF spectrum for the sixth section of the fission plates and the left detector at low bias is given. The data accumulation time is 60 h
Measurements of integral cross sections in the californium-252 fission neutron spectrum
International Nuclear Information System (INIS)
Alberts, W.G.; Guenther, E.; Matzke, M.; Rassl, G.
1977-01-01
In a low-scattering arrangement cross sections averaged over the californium-252 spontaneous fission neutron spectrum were measured. The reactions 27 Al(n,α) 46 Ti, 47 Ti, 48 Ti(n,p), 54 Fe, 56 Fe(n,p), 58 Ni(n,p), 64 Zn(n,p), 115 In(n,n') were studied in order to obtain a consistent set of threshold detectors used in fast neutron flux density measurements. Overall uncertainties between 2 and 2.5% could be achieved; corrections due to neutron scattering in source and samples are discussed
Neutron emission as a probe of fusion-fission and quasi-fission dynamics
International Nuclear Information System (INIS)
Hinde, D.J.
1991-01-01
Pre- and post scission neutron yeilds have been measured as a function of projectile mass, compound nucleus fissility, and fission mass-split and total kinetic energy (TKE) for 27 fusion-fission and quasi-fission reactions induced by beams of 16,18 O, 40 Ar and 64 Ni. A new method of interpretation of experimental pre-scission neutron multiplicities ν-pre and mean kinetic energies ε ν allows the extraction of fission time scales with much less uncertainty than previously, all fusion-fission results being consistent with a dynamical time scale of (35±15) x 10 -21 s for symmetric fission. All reactions show that ν-pre falls quite rapidly with increasing mass-asymmetry; evidence is presented that for fusion-fission reactions this is partly due to a reduction of the dynamical fission time scale with mass-asymmetry. For quasi-fission, the data indicate that the pre-scission multiplicity and mean neutron kinetic energy are very sensitive to the final mass-asymmetry, but that the time scale is virtually independent of mass-asymmetry. It is concluded that for fusion-fission there is no dependence of ν-pre on TKE, whilst for 64 Ni-induced quasi-fission reactions, a strong increase of ν-pre with decreasing TKE is observed, probably largely caused by neutron emission during the acceleration time of the fission fragments in these fast reactions. Interpretation of post-scission multiplicities in terms of fragment excitation energies leads to deduced time scales consistent with those determined from the pre-scission data. 54 refs., 17 tabs., 25 figs
History of the discovery of uranium fission by neutrons
International Nuclear Information System (INIS)
Simane, C.
1989-01-01
The history is briefly described of the discovery of uranium fission by neutrons, based on the texts of original scientific studies, memories or biographies of those who participated in the discovery and of their contemporaries. Obstacles that stood in the way of the discovery are discussed. It is stated that only a few scientists contributed to the discovery of uranium fission. The fission process itself still remains subject of physical research which studies its detailed laws. (Z.M.). 2 tabs., 16 refs
Asymmetry in ternary fission induced by polarized neutrons and fission mechanism
International Nuclear Information System (INIS)
Bunakov, V.E.; Gennenvajn, F.; Dzhessinger, P.; Mutterer, M.; Petrov, G.A.
2003-01-01
The results of measuring the P-odd, P-even (right-left) and T-odd asymmetries of the charged particles emission in the double and ternary fission, induced by the polarized neutrons, are considered. It is shown, what kind of information on the mechanism of the ternary nuclear fission may be obtained from the theoretical analysis of these data [ru
Neutron threshold activation detectors (TAD) for the detection of fissions
Gozani, Tsahi; Stevenson, John; King, Michael J.
2011-10-01
Prompt fission neutrons are one of the strongest signatures of the fission process. Depending on the fission inducing radiation, their average number ranges from 2.5 to 4 neutrons per fission. They are more energetic and abundant, by about 2 orders of magnitude, than the delayed neutrons (≈3 vs. ≈0.01) that are commonly used as indicators for the presence of fissionable materials. The detection of fission prompt neutrons, however, has to be done in the presence of extremely intense probing radiation that stimulated them. During irradiation, the fission stimulation radiation, X-rays or neutrons, overwhelms the neutron detectors and temporarily incapacitate them. Consequently, by the time the detectors recover from the source radiation, fission prompt neutrons are no longer emitted. In order to measure the prompt fission signatures under these circumstances, special measures are usually taken with the detectors such as heavy shielding with collimation, use of inefficient geometries, high pulse height bias and gamma-neutron separation via pulse-shape discrimination with an appropriate organic scintillator. These attempts to shield the detector from the flash of radiation result in a major loss of sensitivity. It can lead to a complete inability to detect the fission prompt neutrons. In order to overcome the blinding induced background from the source radiation, the detection of prompt fission neutrons needs to occur long after the fission event and after the detector has fully recovered from the source overload. A new approach to achieve this is to detect the delayed activation induced by the fission neutrons. The approach demonstrates a good sensitivity in adverse overload situations (gamma and neutron "flash") where fission prompt neutrons could normally not be detected. The new approach achieves the required temporal separation between the detection of prompt neutrons and the detector overload by the neutron activation of the detector material. The technique
Neutron threshold activation detectors (TAD) for the detection of fissions
International Nuclear Information System (INIS)
Gozani, Tsahi; Stevenson, John; King, Michael J.
2011-01-01
Prompt fission neutrons are one of the strongest signatures of the fission process. Depending on the fission inducing radiation, their average number ranges from 2.5 to 4 neutrons per fission. They are more energetic and abundant, by about 2 orders of magnitude, than the delayed neutrons (∼3 vs. ∼0.01) that are commonly used as indicators for the presence of fissionable materials. The detection of fission prompt neutrons, however, has to be done in the presence of extremely intense probing radiation that stimulated them. During irradiation, the fission stimulation radiation, X-rays or neutrons, overwhelms the neutron detectors and temporarily incapacitate them. Consequently, by the time the detectors recover from the source radiation, fission prompt neutrons are no longer emitted. In order to measure the prompt fission signatures under these circumstances, special measures are usually taken with the detectors such as heavy shielding with collimation, use of inefficient geometries, high pulse height bias and gamma-neutron separation via pulse-shape discrimination with an appropriate organic scintillator. These attempts to shield the detector from the flash of radiation result in a major loss of sensitivity. It can lead to a complete inability to detect the fission prompt neutrons. In order to overcome the blinding induced background from the source radiation, the detection of prompt fission neutrons needs to occur long after the fission event and after the detector has fully recovered from the source overload. A new approach to achieve this is to detect the delayed activation induced by the fission neutrons. The approach demonstrates a good sensitivity in adverse overload situations (gamma and neutron 'flash') where fission prompt neutrons could normally not be detected. The new approach achieves the required temporal separation between the detection of prompt neutrons and the detector overload by the neutron activation of the detector material. The technique
Neutron threshold activation detectors (TAD) for the detection of fissions
Energy Technology Data Exchange (ETDEWEB)
Gozani, Tsahi, E-mail: tgozani@rapiscansystems.com [Rapiscan Laboratories, Inc., 520 Almanor Ave., Sunnyvale, CA 94085 (United States); Stevenson, John; King, Michael J. [Rapiscan Laboratories, Inc., 520 Almanor Ave., Sunnyvale, CA 94085 (United States)
2011-10-01
Prompt fission neutrons are one of the strongest signatures of the fission process. Depending on the fission inducing radiation, their average number ranges from 2.5 to 4 neutrons per fission. They are more energetic and abundant, by about 2 orders of magnitude, than the delayed neutrons ({approx}3 vs. {approx}0.01) that are commonly used as indicators for the presence of fissionable materials. The detection of fission prompt neutrons, however, has to be done in the presence of extremely intense probing radiation that stimulated them. During irradiation, the fission stimulation radiation, X-rays or neutrons, overwhelms the neutron detectors and temporarily incapacitate them. Consequently, by the time the detectors recover from the source radiation, fission prompt neutrons are no longer emitted. In order to measure the prompt fission signatures under these circumstances, special measures are usually taken with the detectors such as heavy shielding with collimation, use of inefficient geometries, high pulse height bias and gamma-neutron separation via pulse-shape discrimination with an appropriate organic scintillator. These attempts to shield the detector from the flash of radiation result in a major loss of sensitivity. It can lead to a complete inability to detect the fission prompt neutrons. In order to overcome the blinding induced background from the source radiation, the detection of prompt fission neutrons needs to occur long after the fission event and after the detector has fully recovered from the source overload. A new approach to achieve this is to detect the delayed activation induced by the fission neutrons. The approach demonstrates a good sensitivity in adverse overload situations (gamma and neutron 'flash') where fission prompt neutrons could normally not be detected. The new approach achieves the required temporal separation between the detection of prompt neutrons and the detector overload by the neutron activation of the detector
Cumulative fission yield of Ce-148 produced by thermal-neutron fission of U-235
International Nuclear Information System (INIS)
Hasan, A.A.
1984-12-01
Cumulative fission yield of 148 cesium isotopes and some other fission products produced by thermal-neutron fission of 235 uranium is determined by Germanium/Lithium spectroscopic methods. The measuremets were done at Tsing-Hua open pool reactor using 3 to 4 mg of 93.15% enriched 235 uranium samples. Gamma rays are assigned to the responsible fission products by matching gamma rays energies and half lives. Fission rate is calculated by fission track method. Cumulative fission yields of 148 cesium, 90 krypton, 130 iodine, 144 lanthanum, 89 krypton, 136 xenon, 137 xenon and 140 cesium are calculated. This values are compared with previously predicted values and showed good agreement. 21 Ref
Thermal neutron converter for irradiations with fission neutrons
International Nuclear Information System (INIS)
Wagner, F.M.; Kampfer, S.; Kastenmuller, A.; Waschkowski, W.; Bucherl, Th.; Kampfer, S.
2007-01-01
The new research reactor FRM II at Garching started operation in March 2004. The compact core is cooled by light water, and moderated by heavy water. Two fuel plates mounted in the heavy water tank convert thermal to fast neutrons. The fast neutron flux in the connected beam tube is up to 7 centre dot 10 8 s -1 cm -2 (depending on filters and collimation); the mean neutron energy is about 1.6 MeV. There are two irradiation rooms along the beam. The first is mainly used for medical therapy (MEDAPP facility), the second for materials characterization (NECTAR facility). At the former therapy facility RENT at the old research reactor FRM, the same beam quality was available until July 2000. Therefore, only a small program is run for the determination of the biological effectiveness of the new beam. The neutron and gamma dose rates in the medical beam are 0.54 and 0.20 Gy/min, respectively. The therapy facility MEDAPP is still under examination according to European regulations for medical devices. Full medical operation will start in 2007. The radiography and tomography facility NECTAR is in operation and aims at non-destructive inspection of objects up to 400 kg mass and 80 centre dot 80 centre dot 80 cm 3 in size. As for fission neutrons the macroscopic cross section of hydrogen is much higher than for other materials (e. g. Fe and Pb), one special application is the detection of hydrogen-containing materials (e. g. oil) in dense materials
Energy Technology Data Exchange (ETDEWEB)
Iunes, P J
1990-06-01
Fission track dating is described, focalizing the problem of the decay constant for spontaneous fission of {sup 238} U and the use of neutron dosimetry in fission track analysis. Experimental procedures using thin films of natural uranium as neutron dosimeters and its results are presented. The author shows a intercomparison between different thin films and between the dosimetry with thin film and other dosimetries. (M.V.M.). 52 refs, 12 figs, 9 tabs.
Energy Technology Data Exchange (ETDEWEB)
Billaud, P; Clair, C; Gaudin, M; Genin, R; Joly, R; Leroy, J L; Michaudon, A; Ouvry, J; Signarbieux, C; Vendryes, G [Commissariat a l' Energie Atomique, Saclay (France). Centre d' Etudes Nucleaires
1958-07-01
a) Measurements of neutron induced fission cross-sections in the low energy region. The variation of the fission cross sections of several fissile isotopes has been measured and analysed, for neutron energies below 0,025 eV. The monochromator was a crystal spectrometer used in conjunction with a mechanical velocity selector removing higher order Bragg reflections. The fissile material was laid down on the plates of a fission chamber by painting technic. An ionization chamber, having its plates coated with thin {sup 10}B layers, was used as the neutron flux monitor. b) Measurement of the fission cross section of {sup 235}U. We intend to measure the variation of the neutron induced fission cross section of {sup 235}U over the neutron energy range from 1 keV by the time of flight method. The neutron source is the uranium target of a pulsed 28 MeV electron linear accelerator. The detector is a large fission chamber, with parallel plates, containing about 10 g of {sup 235}U (20 deposits of 25 cm diameter). The relative fission data were corrected for the neutron spectrum measured with a set of BF{sub 3} proportional counters. c) Mean number {nu} of neutrons emitted in neutron induced fission. We measured the value of {nu} for several fissile isotopes in the case of fission induced by 14 MeV neutrons. The 14 MeV neutrons were produced by D (t, n) {alpha} reaction by means of a 300 kV Cockcroft Walton generator. (author)Fren. [French] a) Mesures de sectionficaces de fission a basse energie. Nous avons mesure et analyse la variation de la section efficace de fission de divers isotopes fissiles pour des neutrons d'energie inferieure a 0,025 eV. Le monochromateur est constitue par un spectrometre a cristal auquel est associe un selecteur mecanique destine a eliminer les diffractions de Bragg d'ordre superieur au premier. Le materiau fissile est contenu dans une chambre a fission sous forme de depots realises par peinture; une chambre d'ionisation a depots minces de B{sub 10
Identification of Fissionable Materials Using the Tagged Neutron Technique
International Nuclear Information System (INIS)
Keegan, R.P.; Hurley, J.P.; Tinsley, J.R.; Trainham, R.
2009-01-01
This summary describes experiments to detect and identify fissionable materials using the tagged neutron technique. The objective of this work is to enhance homeland security capability to find fissionable material that may be smuggled inside shipping boxes, containers, or vehicles. The technique distinguishes depleted uranium from lead, steel, and tungsten. Future work involves optimizing the technique to increase the count rate by many orders of magnitude and to build in the additional capability to image hidden fissionable materials. The tagged neutron approach is very different to other techniques based on neutron die-away or photo-fission. This work builds on the development of the Associated Particle Imaging (API) technique at the Special Technologies Laboratory (STL). Similar investigations have been performed by teams at the Oak Ridge National Laboratory (ORNL), the Khlopin Radium Institute in Russia, and by the EURITRACK collaboration in the European Union
Thermal flow in detectors of CNA-II with spontaneous fissions source of 238U
International Nuclear Information System (INIS)
Mascitti, J. A
2012-01-01
The thermal flux in the position of ex-core and in-core CNA-II Nuclear Power Plant (CNA-II) detectors is estimated considering neutron from the 238 U spontaneous fissions as the source, for the reactor cold state (isothermal state with both coolant and moderator at a temperature of 60 o C, a pressure of 35 ata and 15.46 ppm of natural Boron), and 24% inserted control rods (slightly sub-critical). Results are obtained for two different situations: with and without photo-neutrons due to the (γ,n) reaction in D 2 O. It is concluded that the thermal flux is under the detection limit of the boron trifluoride 104-SR or 282-IB detectors (≅10 -1 cm-2.s -1 ). These detectors are located in opposite positions in the inner concrete shielding, having the lowest detection limit among all ex-core detectors. A significant difference is verified in neutron fluxes between both cases, which suggest that photo-neutrons in large heavy water reactors such as CNA-II should not be ignored. The total neutron flux attenuation factor between the inner and outer region of the reactor pressure vessel was estimated to be 7.0 x 10 -7 . It should be mentioned that none of the results here presented has been affected by any correction factor. Each value has a percentage relative error representing the statistical uncertainty due to the probabilistic Monte Carlo method used to obtain it (author)
Neutron and thermal dynamics of a gaseous core fission reactor
International Nuclear Information System (INIS)
van Dam, H.; Kuijper, J.C.; Stekelenburg, A.J.C.; Hoogenboom, J.E.; Boersma-Klein, W.; Kistemaker, J.
1989-01-01
In this paper neutron kinetics and thermal dynamics of a Gaseous Core Fission Reactor with magnetical pumping are shown to have many unconventional aspects. Attention is focused on the properties of the fuel gas, the non-linear neutron kinetics and the energy balance in thermodynamical cycles
Fission decay properties of ultra neutron-rich uranium isotopes
Indian Academy of Sciences (India)
in the chain of neutron-rich uranium isotopes is examined here. The neutron ... mean field theory, this nucleus is shown to undergo exotic decay mode of thermal neu- .... For 250U with a fission barrier of 4.3 MeV [5], we obtain the value of.
Maximum permissible concentration (MPC) values for spontaneously fissioning radionuclides
International Nuclear Information System (INIS)
Ford, M.R.; Snyder, W.S.; Dillman, L.T.; Watson, S.B.
1976-01-01
The radiation hazards involved in handling certain of the transuranic nuclides that exhibit spontaneous fission as a mode of decay were reaccessed using recent advances in dosimetry and metabolic modeling. Maximum permissible concentration (MPC) values in air and water for occupational exposure (168 hr/week) were calculated for 244 Pu, 246 Cm, 248 Cm, 250 Cf, 252 Cf, 254 Cf, /sup 254m/Es, 255 Es, 254 Fm, and 256 Fm. The half-lives, branching ratios, and principal modes of decay of the parent-daughter members down to a member that makes a negligible contribution to the dose are given, and all daughters that make a significant contribution to the dose to body organs following inhalation or ingestion are included in the calculations. Dose commitments for body organs are also given
Backtracing neutron analysis in the fusion-fission dynamics study
International Nuclear Information System (INIS)
Brennand, E. de Goes; Hanappe, F.; Stuttge, L.
2001-01-01
A new method for the analysis of multi parametric experimental data is used in the study of the dynamics of the fission process for the compound system 126 Ba. We apply this method to obtain the correlation between thermal energy related to the neutron total multiplicity and the correlation between pre-scission neutron and pos-scission neutron multiplicities. The results obtained are interpreted into the framework of a dynamical model. From this interpretation we have access to the following information: the friction intensity which drives the dynamical evolution of the system; the initial deformation of the compound system; the barrier evolution with temperature and angular momentum, and fission times. (author)
Micro fission chamber for the ITER neutron monitor
International Nuclear Information System (INIS)
Yamauchi, Michinori; Nishitani, Takeo; Ochiai, Kentaro; Ebisawa, Katsuyuki
2004-01-01
This paper describes the design and the fabrication of a prototype micro-fission chamber and test results under ITER relevant conditions including wide neutron spectrum and intense gamma-rays, and the performance as a ITER power monitor is discussed. A micro-fission chamber with 12 mg UO 2 and a dummy chamber without uranium were designed and fabricated for the in-vessel neutron flux monitoring of ITER. The measurement ability was tested with the FNS facility for 14 MeV neutrons and the 60 Co gamma-ray irradiation facility at JAERI-Takasaki. Employing the Campbelling mode in the electronics, the ITER requirement for the temporal resolution was satisfied. The excellent linearity of the detector output versus the neutron flux was confirmed in the temperature range from 20degC to 250degC. As a result, it was concluded that the developed micro-fission chamber is applicable for ITER. (author)
Study of the number of neutrons produced by fission of 239Pu
International Nuclear Information System (INIS)
Jacob, M.
1958-01-01
Study of the number of neutrons produced by fission of 239 Pu. The counting by coincidence of fissions and neutrons produced by these fissions allows the study of the variation of the mean number of neutrons emitted by ν fission. In the first chapter, it studied the variation of the mean number of neutrons emitted by 239 Pu fission with the energy of the incident neutron. A description of the experiment is given: a spectrometer with a crystal of sodium chloride or beryllium (mounted on a goniometer) is used, a fission chamber containing 10 mg of 239 Pu and the neutron detection system constituted of BF 3 counters which are enriched in 10 B. In the second part, the counting by coincidence of fissions and neutrons produced by the same fission and received by two different groups of counters allow the determination of a relationship between the root mean square and the average of neutron number produced by fission. The variation of the mean number of neutrons emitted by fission of 239 Pu is studied when we change from a thermal spectra of neutrons to a fission spectra of incident neutrons. Finally, when separating in two different part the fission chamber, it is possible to measure the mean number of neutrons emitted from fission of two different sources. It compared the mean number of neutrons emitted by fission of 239 Pu and 233 U. (M.P.)
Energy Technology Data Exchange (ETDEWEB)
Nishio, Katsuhisa; Yamamoto, Hideki; Kimura, Itsuro; Nakagome, Yoshihiro [Kyoto Univ. (Japan)
1997-03-01
Simultaneous measurement of fission fragments and prompt neutrons following the thermal neutron induced fission of U-235 has been performed in order to obtain the neutron multiplicity (v) and its emission energy ({eta}) against the specified mass (m{sup *}) and the total kinetic energy (TKE). The obtained value of -dv/dTKE(m{sup *}) showed a saw-tooth distribution. The average neutron energy <{eta}>(m{sup *}) had a distribution with a reflection symmetry around the half mass division. The measurement also gave the level density parameters of the specified fragment, a(m{sup *}), and this parameters showed a saw-tooth trend too. The analysis by a phenomenological description of this parameters including the shell and collective effects suggested the existence of a collective motion of the fission fragments. (author)
Fission multipliers for D-D/D-T neutron generators
International Nuclear Information System (INIS)
Lou, T.P.; Vujic, J.L.; Koivunoro, H.; Reijonen, J.; Leung, K.-N.
2003-01-01
A compact D-D/D-T fusion based neutron generator is being designed at the Lawrence Berkeley National Laboratory to have a potential yield of 10 12 D-D n/s and 10 14 D-T n/s. Because of its high neutron yield and compact size (∼20 cm in diameter by 4 cm long), this neutron generator design will be suitable for many applications. However, some applications required higher flux available from nuclear reactors and spallation neutron sources operated with GeV proton beams. In this study, a subcritical fission multiplier with k eff of 0.98 is coupled with the compact neutron generators in order to increase the neutron flux output. We have chosen two applications to show the gain in flux due to the use of fission multipliers--in-core irradiation and out-of-core irradiation. For the in-core irradiation, we have shown that a gain of ∼25 can be achieved in a positron production system using D-T generator. For the out-of-core irradiation, a gain of ∼17 times is obtained in Boron Neutron Capture Therapy (BNCT) using a D-D neutron generator. The total number of fission neutrons generated by a source neutron in a fission multiplier with k eff is ∼50. For the out-of-core irradiation, the theoretical maximum net multiplication is ∼30 due to the absorption of neutrons in the fuel. A discussion of the achievable multiplication and the theoretical multiplication will be presented in this paper
Energy Technology Data Exchange (ETDEWEB)
Gautherin, C
1997-09-01
This thesis is devoted to the study of the nuclear structure of neutron-rich nuclei, via the search of isomeric nuclear states. Neutron-rich nuclei were produced in the spontaneous fission of {sup 252}Cf. The experimental study of isomeric states in these nuclei was performed with the {gamma}-array EUROGAM II, coupled to an additional and original fission fragment detector composed by photovoltaic cells, SAPhIR. The photovoltaic cells are well adapted to detect low energy heavy ions and have good energy and time resolutions to obtain a good fission fragment detection. This experiment led to the discovery of new isomeric states in {sup 135}Xe, {sup 104}Mo, {sup 146,147,148}Ce and {sup 152,154,156}Nd, with lifetimes between 60 ns and 2 {mu}s. Level schemes of these nuclei have been completed. An interpretation of the isomeric states in the nuclei {sup 154,156}Nd and {sup 156,158}Sm was performed by Hartree-Fock-Bogolyubov calculations using the DIS Gogny force with two quasi-particles excitations. The confrontation with the experimental results led to an interpretation of these isomeric states as K-isomers. (author)
NECTAR-A fission neutron radiography and tomography facility
International Nuclear Information System (INIS)
Buecherl, T.; Lierse von Gostomski, Ch.; Breitkreutz, H.; Jungwirth, M.; Wagner, F.M.
2011-01-01
NECTAR (Neutron Computerized Tomography and Radiography) is a versatile facility for radiographic and tomographic investigations as well as for neutron activation experiments using fission neutrons. The radiation sources for this facility are two plates of highly enriched uranium situated in the moderator vessel in FRM II. Thermal neutrons originating from the main fuel element of the reactor generate in these plates fast neutrons. These can escape through a horizontal beam tube without moderation. The beam can be filtered and manipulated in order to reduce the accompanying gamma radiation and to match the specific experimental tasks. A summary of the main parameters required for experimental set-up and (quantitative) data evaluation is presented. The (measured) spectra of the neutron and gamma radiations are shown along with the effect of different filters on their behavior. The neutron and gamma fluxes, dose rates, L/D-ratios, etc. and the main parameters of the actually used detection systems for neutron imaging are given, too.
NECTAR-A fission neutron radiography and tomography facility
Energy Technology Data Exchange (ETDEWEB)
Buecherl, T., E-mail: thomas.buecherl@radiochemie.de [Technische Universitaet Muenchen, Lehrstuhl fuer Radiochemie (RCM), Walther-Meissner-Str. 3, 85748 Garching (Germany); Lierse von Gostomski, Ch. [Technische Universitaet Muenchen, Lehrstuhl fuer Radiochemie (RCM), Walther-Meissner-Str. 3, 85748 Garching (Germany); Breitkreutz, H.; Jungwirth, M.; Wagner, F.M. [Technische Universitaet Muenchen, Forschungs-Neutronenquelle Heinz Maier-Leibnitz (FRM II) (Germany)
2011-09-21
NECTAR (Neutron Computerized Tomography and Radiography) is a versatile facility for radiographic and tomographic investigations as well as for neutron activation experiments using fission neutrons. The radiation sources for this facility are two plates of highly enriched uranium situated in the moderator vessel in FRM II. Thermal neutrons originating from the main fuel element of the reactor generate in these plates fast neutrons. These can escape through a horizontal beam tube without moderation. The beam can be filtered and manipulated in order to reduce the accompanying gamma radiation and to match the specific experimental tasks. A summary of the main parameters required for experimental set-up and (quantitative) data evaluation is presented. The (measured) spectra of the neutron and gamma radiations are shown along with the effect of different filters on their behavior. The neutron and gamma fluxes, dose rates, L/D-ratios, etc. and the main parameters of the actually used detection systems for neutron imaging are given, too.
NECTAR—A fission neutron radiography and tomography facility
Bücherl, T.; Lierse von Gostomski, Ch.; Breitkreutz, H.; Jungwirth, M.; Wagner, F. M.
2011-09-01
NECTAR (Neutron Computerized Tomography and Radiography) is a versatile facility for radiographic and tomographic investigations as well as for neutron activation experiments using fission neutrons. The radiation sources for this facility are two plates of highly enriched uranium situated in the moderator vessel in FRM II. Thermal neutrons originating from the main fuel element of the reactor generate in these plates fast neutrons. These can escape through a horizontal beam tube without moderation. The beam can be filtered and manipulated in order to reduce the accompanying gamma radiation and to match the specific experimental tasks. A summary of the main parameters required for experimental set-up and (quantitative) data evaluation is presented. The (measured) spectra of the neutron and gamma radiations are shown along with the effect of different filters on their behavior. The neutron and gamma fluxes, dose rates, L/ D-ratios, etc. and the main parameters of the actually used detection systems for neutron imaging are given, too.
Fission-product yields for thermal-neutron fission of curium-243
International Nuclear Information System (INIS)
Breederland, D.G.
1982-01-01
Cumulative fission yields for 25 gamma rays emitted during the decay of 23 fission products produced by thermal-neutron fission of 243 Cm have been determined. Using Ge(Li) spectroscopy, 33 successive pulse-height spectra of gamma rays emitted from a 77-ng sample of 243 Cm over a period of approximately two and one-half months were analyzed. Reduction of these spectra resulted in the identification and matching of gamma-ray energies and half-lives to specific radionuclides. Using these results, 23 cumulative fission-product yields were calculated. Only those radionuclides having half-lives between 6 hours and 65 days were observed. Prior to this experiment, no fission-product yields had been recorded for 243 Cm
Energy Technology Data Exchange (ETDEWEB)
Davila R, I
1991-06-15
A shielding study is made to attenuate, until maximum permissible levels, the neutrons radiation and photons emitted by spontaneous fission coming from a source of Californium-252. The compound package by a database (Library DLC-23) and the ANISNW code is used, in it version for personal computer. (Author)
Angular distribution in the neutron-induced fission of actinides
Directory of Open Access Journals (Sweden)
Leong L.S.
2013-12-01
Full Text Available Above 1 MeV of incident neutron energy the fission fragment angular distribution (FFAD has generally a strong anisotropic behavior due to the combination of the incident orbital momentum and the intrinsic spin of the fissioning nucleus. This effect has to be taken into account for the efficiency estimation of devices used for fission cross section measurements. In addition it bears information on the spin deposition mechanism and on the structure of transitional states. We designed and constructed a detection device, based on Parallel Plate Avalanche Counters (PPAC, for measuring the fission fragment angular distributions of several isotopes, in particular 232Th. The measurement has been performed at n_TOF at CERN taking advantage of the very broad energy spectrum of the neutron beam. Fission events were recognized by back to back detection in coincidence in two position-sensitive detectors surrounding the targets. The detection efficiency, depending mostly on the stopping of fission fragments in backings and electrodes, has been computed with a Geant4 simulation and validated by the comparison to the measured case of 235U below 3 keV where the emission is isotropic. In the case of 232Th, the result is in good agreement with previous data below 10 MeV, with a good reproduction of the structures associated to vibrational states and the opening of second chance fission. In the 14 MeV region our data are much more accurate than previous ones which are broadly scattered.
Radiography and tomography using fission neutrons at FRM-II
International Nuclear Information System (INIS)
Buecherl, T.; Lierse von Gostomski, Ch.
2004-01-01
Fission neutrons offer complementary information in radiography and tomography compared to the well established techniques using X-rays, gamma-rays, thermal or cold neutrons. They penetrate thick layers of high density materials with only little attenuation, while for light, specially for hydrogen containing materials, their attenuation is high. In the past, fast neutrons for NDT (non-destructive testing) were only available at accelerator driven systems. These high energy neutrons have to be moderated to achieve acceptable detection efficiencies thus drastically reducing the available neutron intensities and either resulting in a high beam divergence or in additional losses in neutron intensities due to beam collimation. The recently installed neutron computerized tomography and radiography system NECTAR at the Forschungsreaktor Muenchen-II (FRM-II) overcomes these disadvantages by using fission neutrons of about 1.7 MeV mean energy created in two converter plates set-up of highly enriched uranium. The beam quality, i.e. the neutron divergence can be adapted to the object to be measured by using different collimators, resulting in L/D-values up to 300. The available neutron beam intensity at the measuring position is up to 1.7E+08 cm -2 s -1 for a maximum beam area of 40 cm x 40 cm. For conventional imaging a two-dimensional detector system based on a CCD-camera is used, other more specialised systems are available. (author)
Radiography and tomography using fission neutrons at FRM-II
Energy Technology Data Exchange (ETDEWEB)
Buecherl, T.; Lierse von Gostomski, Ch. [Inst. fuer Radiochemie, TU-Muenchen, Garching (Germany)
2004-07-01
Fission neutrons offer complementary information in radiography and tomography compared to the well established techniques using X-rays, gamma-rays, thermal or cold neutrons. They penetrate thick layers of high density materials with only little attenuation, while for light, specially for hydrogen containing materials, their attenuation is high. In the past, fast neutrons for NDT (non-destructive testing) were only available at accelerator driven systems. These high energy neutrons have to be moderated to achieve acceptable detection efficiencies thus drastically reducing the available neutron intensities and either resulting in a high beam divergence or in additional losses in neutron intensities due to beam collimation. The recently installed neutron computerized tomography and radiography system NECTAR at the Forschungsreaktor Muenchen-II (FRM-II) overcomes these disadvantages by using fission neutrons of about 1.7 MeV mean energy created in two converter plates set-up of highly enriched uranium. The beam quality, i.e. the neutron divergence can be adapted to the object to be measured by using different collimators, resulting in L/D-values up to 300. The available neutron beam intensity at the measuring position is up to 1.7E+08 cm{sup -2} s{sup -1} for a maximum beam area of 40 cm x 40 cm. For conventional imaging a two-dimensional detector system based on a CCD-camera is used, other more specialised systems are available. (author)
On angular distribution of nucleus fission fragments by fast neutrons
International Nuclear Information System (INIS)
Barabanov, A.L.; Grechukhin, D.P.
1987-01-01
Evaluation of amplitudes of quadrupole and hexadecapole components of angular distribution of nucleus fission fragments by neutrons with the energies E n < or approx. 6 MeV is conducted. Stability of this amplitude to permeability optical coefficient variations for neutrons is revealed. It is shown, that the ratio of these amplitudes as well as the character of their dependence on the target nucleus orientation degree are sensitive to the type of fission probability distribution along K projection if fissile nucleus J spin to the fragment scattering axis. This sensitivity may be used for fragment angular distribution anisotropy formation statistical model verification
Fission meter and neutron detection using poisson distribution comparison
Rowland, Mark S; Snyderman, Neal J
2014-11-18
A neutron detector system and method for discriminating fissile material from non-fissile material wherein a digital data acquisition unit collects data at high rate, and in real-time processes large volumes of data directly into information that a first responder can use to discriminate materials. The system comprises counting neutrons from the unknown source and detecting excess grouped neutrons to identify fission in the unknown source. Comparison of the observed neutron count distribution with a Poisson distribution is performed to distinguish fissile material from non-fissile material.
8-group relative delayed neutron yields for monoenergetic neutron induced fission of 239Pu
International Nuclear Information System (INIS)
Piksaikin, V.M.; Kazakov, L.E.; Isaev, S.G.; Korolev, G.G.; Roshchenko, V.A.; Tertychnyj, R.G
2002-01-01
The energy dependence of the relative yield of delayed neutrons in an 8-group model representation was obtained for monoenergetic neutron induced fission of 239 Pu. A comparison of this data with the available experimental data by other authors was made in terms of the mean half-life of the delayed neutron precursors. (author)
Effect of fission dynamics on the spectra and multiplicities of prompt fission neutrons
International Nuclear Information System (INIS)
Nix, J.R.; Madland, D.G.; Sierk, A.J.
1985-01-01
With the goal of examining their effect on the spectra and multiplicities of the prompt neutrons emitted in fission, we discuss recent advances in a unified macroscopic-microscopic description of large-amplitude collective nuclear dynamics. The conversion of collective energy into single-particle excitation energy is calculated for a new surface-plus-window dissipation mechanism. By solving the Hamilton equations of motion for initial conditions appropriate to fission, we obtain the average fission-fragment translational kinetic energy and excitation energy. The spectra and multiplicities of the emitted neutrons, which depend critically upon the average excitation energy, are then calculated on the basis of standard nuclear evaporation theory, taking into account the average motion of the fission fragments, the distribution of fission-fragment residual nuclear temperature, the energy dependence of the cross section for the inverse process of compound-nucleus formation, and the possibility of multiple-chance fission. Some illustrative comparisons of our calculations with experimental data are shown
International Nuclear Information System (INIS)
Korotkin, Yu.S.; Ter-Akop'yan, G.M.; Popeko, A.G.; Drobina, T.P.; Zhuravleva, E.L.
1982-01-01
The results of experiments on further concentration of a new natural spontaneously fissionable nuclide, the concentrates of which form the Cheleken geothermal brines have been obtained, are presented. The conclusions are drown about the chemical nature of a new spontaneously fissionable nuclide. It is a chalcophile element which copreipitates with sulphides of copper, lead, arsenic and mercury from weakly acid solutions. The behaviour of the new nuclide in sulphide systems in many respects is similar to the behaviour of polonium, astatine and probably of bismuth. The most probable stable valence of the new nuclide varies from +1 up to +3. The data available on the chemical behaviour of the new nuclide as well as the analysis over contamination by spontaneously fissionable isotopes permit to state that the new natural spontaneously fissionable nuclide does not relate to the known isotopes
Neutron kinetics in moderators and SNM detection through epithermal-neutron-induced fissions
Energy Technology Data Exchange (ETDEWEB)
Gozani, Tsahi, E-mail: tgmaven@gmail.com [1050 Harriet St., Palo Alto, CA 94301 (United States); King, Michael J. [Rapiscan Laboratories Inc., 520 Almanor Ave., Sunnyvale, CA 94085 (United States)
2016-01-01
Extension of the well-established Differential Die Away Analysis (DDAA) into a faster time domain, where more penetrating epithermal neutrons induce fissions, is proposed and demonstrated via simulations and experiments. In the proposed method the fissions stimulated by thermal, epithermal and even higher-energy neutrons are measured after injection of a narrow pulse of high-energy 14 MeV (d,T) or 2.5 MeV (d,D) source neutrons, appropriately moderated. The ability to measure these fissions stems from the inherent correlation of neutron energy and time (“E–T” correlation) during the process of slowing down of high-energy source neutrons in common moderating materials such as hydrogenous compounds (e.g., polyethylene), heavy water, beryllium and graphite. The kinetic behavior following injection of a delta-function-shaped pulse (in time) of 14 MeV neutrons into such moderators is studied employing MCNPX simulations and, when applicable, some simple “one-group” models. These calculations served as a guide for the design of a source moderator which was used in experiments. Qualitative relationships between slowing-down time after the pulse and the prevailing neutron energy are discussed. A laboratory system consisting of a 14 MeV neutron generator, a polyethylene-reflected Be moderator, a liquid scintillator with pulse-shape discrimination (PSD) and a two-parameter E–T data acquisition system was set up to measure prompt neutron and delayed gamma-ray fission signatures in a 19.5% enriched LEU sample. The measured time behavior of thermal and epithermal neutron fission signals agreed well with the detailed simulations. The laboratory system can readily be redesigned and deployed as a mobile inspection system for SNM in, e.g., cars and vans. A strong pulsed neutron generator with narrow pulse (<75 ns) at a reasonably high pulse frequency could make the high-energy neutron induced fission modality a realizable SNM detection technique.
Neutron emission and fragment yield in high-energy fission
International Nuclear Information System (INIS)
Grudzevich, O. T.; Klinov, D. A.
2013-01-01
The KRIS special library of spectra and emission probabilities in the decays of 1500 nuclei excited up to energies between 150 and 250 MeV was developed for correctly taking into account the decay of highly excited nuclei appearing as fission fragments. The emission of neutrons, protons, and photons was taken into account. Neutron emission fromprimary fragments was found to have a substantial effect on the formation of yields of postneutron nuclei. The library was tested by comparing the calculated and measured yields of products originating from the fission of nuclei that was induced by high-energy protons. The method for calculating these yields was tested on the basis of experimental data on the thermal-neutroninduced fission of 235 U nuclei
Neutronics issues in fusion-fission hybrid reactor design
International Nuclear Information System (INIS)
Liu Chengan
1995-01-01
The coupled neutron and γ-ray transport equations and nuclear number density equations, and its computer program systems concerned in fusion-fission hybrid reactor design are briefly described. The current status and focal point for coming work of nuclear data used in fusion reactor design are explained
Analytic computation of average energy of neutrons inducing fission
International Nuclear Information System (INIS)
Clark, Alexander Rich
2016-01-01
The objective of this report is to describe how I analytically computed the average energy of neutrons that induce fission in the bare BeRP ball. The motivation of this report is to resolve a discrepancy between the average energy computed via the FMULT and F4/FM cards in MCNP6 by comparison to the analytic results.
Disintegration constant of uranium-238 by spontaneous fission redetermined by glass track method
International Nuclear Information System (INIS)
Lima Medeiros, E. de.
1978-01-01
The disintegration constant of U 238 by spontaneous fission using glass as fission fragment detector was redetermined. A film of natural uranium (UO 3 ) prepared by chemical methods on the glass lamina was used in a long time experience of exposure (about 16 years). The good conditions of sample preparation and storage allow to observe, after chemical etching, fission fragment tracks. (M.C.K.) [pt
Neutron-nucleus interactions and fission. Chapter 1
International Nuclear Information System (INIS)
1998-01-01
The central problem in nuclear-reactor kinetics is to predict the evolution in time of the neutron population in a multiplying medium. Point kinetics allows study of the global behaviour of the neutron population from the average properties of the medium. Before tackling, in the following chapters, the equations governing the time variation of the reactor power (proportional to the total neutron population), the properties of a neutron-multiplying medium shall be discussed briefly. After recalling a number of definitions, a qualitative description shall be given of the principal nuclear reactions at play in a self-sustaining chain reaction, with emphasis on the source of fission neutrons. Since delayed neutrons play a crucial role in reactor kinetics, their production in a reactor shall be described in greater detail. (author)
MADNIX a code to calculate prompt fission neutron spectra and average prompt neutron multiplicities
International Nuclear Information System (INIS)
Merchant, A.C.
1986-03-01
A code has been written and tested on the CDC Cyber-170 to calculate the prompt fission neutron spectrum, N(E), as a function of both the fissioning nucleus and its excitation energy. In this note a brief description of the underlying physical principles involved and a detailed explanation of the required input data (together with a sample output for the fission of 235 U induced by 14 MeV neutrons) are presented. Weisskopf's standard nuclear evaporation theory provides the basis for the calculation. Two important refinements are that the distribution of fission-fragment residual nuclear temperature and the cooling of the fragments as neutrons are emitted approximately taken into account, and also the energy dependence of the cross section for the inverse process of compound nucleus formation is included. This approach is then used to calculate the average number of prompt neutrons emitted per fission, v-bar p . At high excitation energies, where fission is still possible after neutron emission, the consequences of the competition between first, second and third chance fission on N(E) and v-bar p are calculated. Excellent agreement with all the examples given in the original work of Madland and Nix is obtained. (author) [pt
Ternary Fission of U235 by Resonance Neutrons
International Nuclear Information System (INIS)
Kvitek, I.; Popov, Ju.P.; Rjabov, Ju.V.
1965-01-01
Recently a number of papers have appeared indicating considerable variations in the ratio of the ternary-fission cross-section to the binary-fission cross-section of U 235 on transition from one neutron resonance to another. However, such variations have not been discovered in U 233 and Pu 239 . The paper reports investigations of the ternary fission of U 235 by neutrons with an energy of 0.1 to 30 eV. Unlike other investigators of the ternary fission of U 235 , we identified the ternary-fission event by the coincidence of one of the fission fragments with a light long-range particle. This made it passible to separate ternary fissions from the possible contribution of the (n, α)reaction. The measurements were performed at the fast pulsed reactor of the Joint Institute for Nuclear Research by the time-of-flight method. A flight length of 100 m was used, giving a resolution of 0.6 μs/m. Gas scintillation counters filled with xenon at a pressure of 2 atm were used to record the fission fragments and the light long-range particle. A layer of enriched U 235 ∼2 mg/cm 2 thick and ∼300 cm 2 in area was applied to an aluminium foil 20-fim thick. The scintillations from the fission fragments were recorded in the gas volume on one side of the foil and those from the light long-range particles in that on the other. In order to assess the background (e.g . coincidences of the pulse from a fragment with that from a fission gamma quantum or a proton from the (n, p) reaction in the aluminium foil), a measurement was carried out in which the volume recording the long-range particle was shielded with a supplementary aluminium filter 1-mm thick. The results obtained indicate the absence of the considerable variations in the ratio between the ternary-and binary- fission cross-sections for U 235 that have been noted by other authors. Measurements showed no irregularity in the ratio of the cross-sections in the energy range 0.1 to 0.2 eV. The paper discusses the possible effect of
Gatera, Angélique; Göök, Alf; Hambsch, Franz-Josef; Moens, André; Oberstedt, Andreas; Oberstedt, Stephan; Sibbens, Goedele; Vanleeuw, David; Vidali, Marzio
2018-03-01
Recent years have seen an increased interest in prompt fission γ-ray (PFG) measurements motivated by a high priority request of the OECD/NEA for high precision data, mainly for the nuclear fuel isotopes 235U and 239Pu. Our group has conducted a PFG measurement campaign using state-of-the-art lanthanum halide detectors for all the main actinides to a precision better than 3%. The experiments were performed in a coincidence setup between a fission trigger and γ-ray detectors. The time-of-flight technique was used to discriminate photons, traveling at the speed of light, and prompt fission neutrons. For a full rejection of all neutrons below 20 MeV, the PFG time window should not be wider than a few nanoseconds. This window includes most PFG, provided that no isomeric states were populated during the de-excitation process. When isomeric states are populated, PFGs can still be emitted up to 1 yus after the instant of fission or later. To study these γ-rays, the detector response to neutrons had to be determined and a correction had to be applied to the γ-ray spectra. The latest results for PFG characteristics from the reaction 239Pu(nth,f) will be presented, together with an analysis of PFGs emitted up to 200 ns after fission in the spontaneous fission of 252Cf as well as for thermal-neutron induced fission on 235U and 239Pu. The results are compared with calculations in the framework of the Hauser-Feshbach Monte Carlo code CGMF and FIFRELIN.
Recent developments on micrometric fission chambers for high neutron fluxes
International Nuclear Information System (INIS)
Letourneau, A.; Bringer, O.; Dupont, E.; Marie, F.; Panebianco, S.; Toussaint, J. C.; Veyssiere, C.; Chabod, S.; Breaud, S.; Oriol, L.
2009-01-01
With the development of innovative nuclear systems and new generation neutron sources, the nuclear instrumentation should be adapted. Since several years, we developed microscopic fission chambers to study the transmutation of minor actinides in high thermal-neutron fluxes. The recent developments done to fulfill the drastic conditions of irradiations are described in this paper together with the feedback from the measurements. Two installations were used: the HFR of the ILL for its highest thermal neutron flux of the world and the MEGAPIE target which was the first 1 MW liquid Pb-Bi spallation target in the world. (authors)
Recent developments on micrometric fission chambers for high neutron fluxes
Energy Technology Data Exchange (ETDEWEB)
Letourneau, A. [Irfu, Service de Physique Nucleaire, CEA-Saclay, 91191 Gif-sur-Yvette (France); Bringer, O.; Dupont, E.; Marie, F.; Panebianco, S.; Toussaint, J. C.; Veyssiere, C. [Irfu, CEA-Saclay, 91191 Gif-sur-Yvette (France); Chabod, S. [LPSC, Universite Joseph Fourier Grenoble 1, CNRS/IN2P3 (France); Breaud, S.; Oriol, L. [DEN/DER/SPEX, CEA-Cadarache, Saint-Paul-lez-Durances (France)
2009-07-01
With the development of innovative nuclear systems and new generation neutron sources, the nuclear instrumentation should be adapted. Since several years, we developed microscopic fission chambers to study the transmutation of minor actinides in high thermal-neutron fluxes. The recent developments done to fulfill the drastic conditions of irradiations are described in this paper together with the feedback from the measurements. Two installations were used: the HFR of the ILL for its highest thermal neutron flux of the world and the MEGAPIE target which was the first 1 MW liquid Pb-Bi spallation target in the world. (authors)
International Nuclear Information System (INIS)
Nicoli, I.G.
1981-06-01
A radiochemical investigation is performed to measure the cumulative fission product yields of several lantanides and yttrium nuclides in the 238 U by fission neutron spectra. Natural and depleted uranium are irradiated under the same experimental conditions in order to find a way to subtract the contribution of the 235 U fission. 235 U percentage in the natural uranium was 3.5 times higher than in the depleted uranium. Uranium oxides samples are irradiated inside the core of the Argonaut Reactor, at the Instituto de Engenharia Nuclear, and the lantanides and yttrium are chemically separated. The fission products gamma activities were detected, counted and analysed in a system constituted by a high resolution Ge(Li) detector, 4096 multichannel analyser and a PDP-11 computer. Cumulative yields for fission products with half-lives between 1 to 33 hours are measured: 93 Y, 141 La, 142 La, 143 Ce and 149 Nd. The chain total yields are calculated. The cumulative fission yields measured for 93 Y, 141 La, 142 La, 143 Ce and 149 Nd are 4,49%, 4,54%, 4,95%, 4,16% and 1,37% respectively and they are in good agreement with the values found in the literature. (Author) [pt
Uranium borehole logging using delayed or prompt fission neutrons
International Nuclear Information System (INIS)
Schulze, G.; Wuerz, H.
1977-04-01
The measurement of induced fission neutrons using Cf 252 and 14 MeV neutrons is a sensitive method for an in situ determination of Uranium. Applying this methods requires a unique relation between concentration of Uranium and intensity of induced fission neutrons. A discussion of parameters influencing the determination of concentration is given. A simple method is developed allowing an elemination of the geochemistry of the deposit and of the borehole configuration. Borehole probes using the methods described are of considerable help during the phase of detailed exploration of uranium ore deposits. These on-line tools allow an immediate determination of concentration. Thus avoiding the expensive and time consuming step of core drilling and subsequent chemical analysis. (orig./HP) [de
Neutron irradiation facilities for fission and fusion reactor materials studies
International Nuclear Information System (INIS)
Rowcliffe, A.F.
1985-01-01
The successful development of energy-conversion machines based upon nuclear fission or fusion reactors is critically dependent upon the behavior of the engineering materials used to construct the full containment and primary heat extraction systems. The development of radiation damage-resistant materials requires irradiation testing facilities which reproduce, as closely as possible, the thermal and neutronic environment expected in a power-producing reactor. The Oak Ridge National Laboratory (ORNL) reference core design for the Center for Neutron Research (CNR) reactor provides for instrumented facilities in regions of both hard and mixed neutron spectra, with substantially higher fluxes than are currently available. The benefits of these new facilities to the development of radiation damage resistant materials are discussed in terms of the major US fission and fusion reactor programs
International Nuclear Information System (INIS)
Yanjushkin, V.A.
1991-01-01
At developing new methods of non-destructive determination of plutonium full mass in nuclear materials and products being involved in uranium -plutonium fuel cycle by its intrinsic neutron radiation, it may be useful to know not only separate moments but the multiplicity distribution law itself of neutron leaving this material surface using the following as parameters - firstly, unconditional multiplicity distribution laws of neutrons formed in spontaneous and induced fission acts of the given fissionable material corresponding nuclei and unconditional multiplicity distribution law of neutrons caused by (α,n) reactions at light nuclei of some elements which compose this material chemical structure; -secondly, probability of induced fission of this material nuclei by an incident neutron of any nature formed during the previous fissions or(α,n) reactions. An attempt to develop similar theory has been undertaken. Here the author proposes his approach to this problem. The main advantage of this approach, to our mind, consists in its mathematical simplicity and easy realization at the computer. In principle, the given model guarantees any good accuracy at any real value of induced fission probability without limitations dealing with physico-chemical composition of nuclear material
Yields of fission products produced by thermal-neutron fission of 229Th
International Nuclear Information System (INIS)
Dickens, J.K.; McConnell, J.W.
1983-01-01
Absolute yields have been determined for 47 gamma rays emitted in the decay of 37 fission products representing 25 mass chains created during thermal-neutron fission of 229 Th. Using a Ge(Li) detector, spectra were obtained of gamma rays emitted between 15 min and 0.4 yr after very short irradiations by thermal neutrons of a 15-μg sample of 229 Th. On the basis of measured gamma-ray yields and known nuclear data, yields for cumulative production of 37 fission products were deduced. The absolute overall normalization uncertainty is 235 U, we postulate a simple functional dependence sigma = sigma(Z/sub p/), and using this dependence obtain values of Z/sub p/(A) for 15 mass chains created during fission of 229 Th. Values of Z/sub p/(A) were estimated for other mass chains based upon results of a recent study of Z/sub p/(A). Charge distributions determined using the deduced mass distribution and the deduced sets of Z/sub p/(A) and sigma(Z/sub p/) are in very good agreement with recent measurements, exhibiting a pronounced even-odd effect in elemental yields. These results may be used to predict unmeasured yields for 229 Th fission
Differential and integral characteristics of prompt fission neutrons in the statistical theory
International Nuclear Information System (INIS)
Gerasimenko, B.F.; Rubchenya, V.A.
1989-01-01
Hauser-Feshbach statistical theory is the most consistent approach to the calculation of both spectra and prompt fission neutrons characteristics. On the basis of this approach a statistical model for calculation of differential prompt fission neutrons characteristics of low energy fission has been proposed and improved in order to take into account the anisotropy effects arising at prompt fission neutrons emission from fragments. 37 refs, 6 figs
Progress in fission product nuclear data
International Nuclear Information System (INIS)
Lammer, M.
1984-09-01
This is the tenth issue of a report series on Fission Product Data, which informs us about all the activities in this field, which are planned, ongoing, or have recently been completed. The types of activities included are measurements, compilations and evaluations of: fission product yields (neutron induced and spontaneous fission), neutron reaction cross sections of fission products, data related to the radioactive decay of fission products, delayed neutron data of fission products, lumped fission product data (decay heat, absorption, etc.). There is also a section with recent references relative to fission product nuclear data
International Nuclear Information System (INIS)
Prosdocimi, A.
1979-01-01
A method for determining the absolute reaction rate of nuclear events giving rise to neutron emission, according to their neutron multiplicity, is proposed. A typical application is the measurement of the (α, n) and spontaneous fission rates in a fissile material sample, particularly of Pu oxide composition. An analysis of random and correlated neutron pulses is carried out on the basis of sequential order without requiring any time interval analysis, then the primary nuclear events are sorted versus their neutron multiplicity. Suitable theoretical relationships enable to derive the absolute (α, n) and SF reaction rates when the physical parameters of the neutron detector and the multiplicity spectrumm of pulses are known. A typical device is described and the results of experiments leading to Pu-239 and Pu-240 assay are given
Fission neutrons experiments, evaluation, modeling and open problems
Kornilov, Nikolay
2014-01-01
Although the fission of heavy nuclei was discovered over 75 years ago, many problems and questions still remain to be addressed and answered. The reader will be presented with an old, but persistent problem of this field: The contradiction between Prompt Fission Neutron (PFN) spectra measured with differential (microscopic) experiments and integral (macroscopic and benchmark) experiments (the Micro-Macro problem). The difference in average energy is rather small ~3% but it is stable and we cannot explain the difference due to experimental uncertainties. Can we measure the PFN spectrum with hig
Fission and activation of uranium by fashion-plasma neutrons
International Nuclear Information System (INIS)
Lee, J.H.; Hochl, F.; McFarland, D.R.
1978-01-01
Disks of enriched and depleted uranium were irradiated by neutrons from the D-D fusions in a dense plasma-focus. A fission yield of 10 6 fissions-cm -3 in U 235 per pulse was determined with Ge(Li) gamme-ray spectrometry. Activation of U 238 caused increased beta activity after the plasma-neutron irradiation but alpha-particle spectrometry showed Pu 239 production was negligible. In addition, with a disk of lithium in the apparatus, 13.3 MeV neutrons from 7 Li(d,n) 8 Be was observed with a 80-m time-of-flight neutron detector. Dense plasma focuses are now operated not only in a single coaxial gun, but also in improved geometries, such as the hypocycloidal pinch and the staged plasma focus, from which a multiple plasma-focus array suitable for experimental verification of, and eventuel development into a fusion-fission hybrid reactor could be produced. (orig.) [de
Laurec, J.; Adam, A.; de Bruyne, T.; Bauge, E.; Granier, T.; Aupiais, J.; Bersillon, O.; Le Petit, G.; Authier, N.; Casoli, P.
2010-12-01
The yields of more than fifteen fission products have been carefully measured using radiochemical techniques, for 235U(n,f), 239Pu(n,f) in a thermal spectrum, for 233U(n,f), 235U(n,f), and 239Pu(n,f) reactions in a fission neutron spectrum, and for 233U(n,f), 235U(n,f), 238U(n,f), and 239Pu(n,f) for 14.7 MeV monoenergetic neutrons. Irradiations were performed at the EL3 reactor, at the Caliban and Prospero critical assemblies, and at the Lancelot electrostatic accelerator in CEA-Valduc. Fissions were counted in thin deposits using fission ionization chambers. The number of fission products of each species were measured by gamma spectrometry of co-located thick deposits.
International Nuclear Information System (INIS)
Anon.
1975-01-01
The nuclear fission research programs are designed to elucidate basic features of the fission process. Specifically, (1) factors determining how nucleons of a fissioning nucleus are distributed between two fission fragments, (2) factors determining kinetic energy and excitation energies of fragments, and (3) factors controlling fission lifetimes. To these ends, fission studies are reported for several heavy elements and include investigations of spontaneous and neutron-induced fission, heavy ion reactions, and high energy proton reactions. The status of theoretical research is also discussed. (U.S.)
Actinide neutron-induced fission up to 20 MeV
International Nuclear Information System (INIS)
Maslov, V.M.
2001-01-01
Fission and total level densities modelling along with double-humped fission barrier parameters allow to describe available actinide neutron-induced fission cross section data in the incident neutron energy range of ∼ 10 keV - 20 MeV. Saddle asymmetries relevant to shell correction model calculations influence fission barriers, extracted by cross section data analysis. The inner barrier was assumed axially symmetric in case of U, Np and Pu neutron-deficient nuclei. It is shown that observed irregularities in neutron-induced fission cross section data in the energy range of 0.5-3 MeV could be attributed to the interplay of few-quasiparticle excitations in the level density of fissioning and residual nuclei. Estimates of first-chance fission cross section and secondary neutron spectrum model were validated by 238 U fission, (n,2n) and (n,3n) data description up to 20 MeV. (author)
Actinide neutron-induced fission up to 20 MeV
Energy Technology Data Exchange (ETDEWEB)
Maslov, V M [Radiation Physics and Chemistry Problems Institute, Minsk-Sosny (Belarus)
2001-12-15
Fission and total level densities modelling along with double-humped fission barrier parameters allow to describe available actinide neutron-induced fission cross section data in the incident neutron energy range of {approx} 10 keV - 20 MeV. Saddle asymmetries relevant to shell correction model calculations influence fission barriers, extracted by cross section data analysis. The inner barrier was assumed axially symmetric in case of U, Np and Pu neutron-deficient nuclei. It is shown that observed irregularities in neutron-induced fission cross section data in the energy range of 0.5-3 MeV could be attributed to the interplay of few-quasiparticle excitations in the level density of fissioning and residual nuclei. Estimates of first-chance fission cross section and secondary neutron spectrum model were validated by {sup 238}U fission, (n,2n) and (n,3n) data description up to 20 MeV. (author)
Yields of fission products produced by thermal-neutron fission of 245Cm
International Nuclear Information System (INIS)
Dickens, J.K.; McConnell, J.W.
1981-01-01
Absolute yields have been determined for 105 gamma rays emitted in the decay of 95 fission products representing 54 mass chains created during thermal-neutron fission of 245 Cm. These results include 17 mass chains for which no prior yield data exist. Using a Ge(Li) detector, spectra were obtained of gamma rays between 30 sec and 0.3 yr after very short irradiations of thermal neutrons on a 1 μg sample of 245 Cm. On the basis of measured gamma-ray yields and known nuclear data, total chain mass yields and relative uncertainties were obtained for 51 masses between 84 and 156. The absolute overall normalization uncertainty is 239 Pu and for 252 Cf(s.f.); the influences of the closed shells Z=50, N=82 are not as marked as for thermal-neutron fission of 239 Pu but much more apparent than for 252 Cf(s.f.). Information on the charge distribution along several isobaric mass chains was obtained by determining fractional yields for 12 fission products. The charge distribution width parameter, based upon data for the heavy masses, A=128 to 140, is independent of mass to within the uncertainties of the measurements. Gamma-ray assignments were made for decay of short-lived fission products for which absolute gamma-ray transition probabilities are either not known or in doubt. Absolute gamma-ray transition probabilities were determined as (51 +- 8)% for the 374-keV gamma ray from decay of 110 Rh, (35 +- 7)% for the 1096-keV gamma ray from decay of 133 Sb, and (21.2 +- 1.2)% for the 255-keV gamma ray from decay of 142 Ba
Delayed neutrons as a probe of nuclear charge distribution in fission of heavy nuclei by neutrons
Isaev, S G; Piksaikin, V M; Roshchenko, V A
2001-01-01
A method of the determination of cumulative yields of delayed neutron precursors is developed. This method is based on the iterative least-square procedure applied to delayed neutron decay curves measured after irradiation of sup 2 sup 3 sup 5 U sample by thermal neutrons. Obtained cumulative yields in turns were used for deriving the values of the most probable charge in low-energy fission of the above-mentioned nucleus.
Delayed neutrons as a probe of nuclear charge distribution in fission of heavy nuclei by neutrons
International Nuclear Information System (INIS)
Isaev, S.G.; Piksaikin, V.M.; Kazakov, L.E.; Roshchenko, V.A.
2002-01-01
A method of the determination of cumulative yields of delayed neutron precursors is developed. This method is based on the iterative least-square procedure applied to delayed neutron decay curves measured after irradiation of 235 U sample by thermal neutrons. Obtained cumulative yields in turns were used for deriving the values of the most probable charge in low-energy fission of the above-mentioned nucleus. (author)
Yields of fission products produced by thermal-neutron fission of 249Cf
International Nuclear Information System (INIS)
Dickens, J.K.; McConnell, J.W.
1981-01-01
Absolute yields have been determined for 107 gamma rays emitted in the decay of 97 fission products representing 54 mass chains created during thermal-neutron fission of 249 Cf. These results include 14 mass chains for which no prior yield data exist. Using a Ge(Li) detector, spectra were obtained of gamma rays emanating from a 0.4 μg sample of 249 Cf between 45 s and 0.4 yr after very short irradiations of the 249 Cf by thermal neutrons. On the basis of measured gamma-ray yields and known nuclear data, total chain mass yields and relative uncertainties were obtained for 51 masses between 89 and 156. The absolute overall normalization uncertainty is approx.8%. The measured A-chain cumulative yields make up 77% of the total light mass (A 249 Cf
What can be learnt from the channel analysis of the 232Th neutron fission cross section
International Nuclear Information System (INIS)
Abou Yehia, H.; Jary, J.; Trochon, J.; Boldeman, J.W.; Musgrove, A.R. de L.
1979-10-01
Channel analyses of the neutron fission cross section of 232 Th have been made in two laboratories. The calculated fission cross sections and fission fragment anisotropies are compared with the experimental data. Despite some differences in the methods used, the conclusions on the physical aspects of the fission process are very similar
Design of ITER neutron monitor using micro fission chambers
International Nuclear Information System (INIS)
Nishitani, Takeo; Ebisawa, Katsuyuki; Ando, Toshiro; Kasai, Satoshi; Johnson, L.C.; Walker, C.
1998-08-01
We are designing micro fission chambers, which are pencil size gas counters with fissile material inside, to be installed in the vacuum vessel as neutron flux monitors for ITER. We found that the 238 U micro fission chambers are not suitable because the detection efficiency will increase up to 50% in the ITER life time by breading 239 Pu. We propose to install 235 U micro fission chambers on the front side of the back plate in the gap between adjacent blanket modules and behind the blankets at 10 poloidal locations. One chamber will be installed in the divertor cassette just under the dome. Employing both pulse counting mode and Campbelling mode in the electronics, we can accomplish the ITER requirement of 10 7 dynamic range with 1 ms temporal resolution, and eliminate the effect of gamma-rays. We demonstrate by neutron Monte Carlo calculation with three-dimensional modeling that we avoid those detection efficiency changes by installing micro fission chambers at several poloidal locations inside the vacuum vessel. (author)
Neutron Induced Capture and Fission Processes on 238U
Directory of Open Access Journals (Sweden)
Oprea Cristiana
2016-01-01
Full Text Available Nuclear data on Uranium isotopes are of crucial interest for new generation of nuclear reactors. Processes of interest are the nuclear reactions induced by neutrons and in this work mainly the capture and the fission process on 238U will be analyzed in a wide energy interval. For slow and resonant neutrons the many levels Breit – Wigner formalism is necessary. In the case of fast and very fast neutrons up to 200 MeV the nuclear reaction mechanism implemented in Talys will be used. The present evaluations are necessary in order to obtain the field of neutrons in the design of nuclear reactors and they are compared with experimental data from literature obtained from capture and (n,xn processes.
Delayed neutron spectra from short pulse fission of uranium-235
International Nuclear Information System (INIS)
Atwater, H.F.; Goulding, C.A.; Moss, C.E.; Pederson, R.A.; Robba, A.A.; Wimett, T.F.; Reeder, P.; Warner, R.
1986-01-01
Delayed neutron spectra from individual short pulse (∼50 μs) fission of small 235 U samples (50 mg) were measured using a small (5 cm OD x 5 cm length) NE 213 neutron spectrometer. The irradiating fast neutron flux (∼10 13 neutrons/cm 2 ) for these measurements was provided by the Godiva fast burst reactor at the Los Alamos Critical Experiment Facility (LACEF). A high speed pneumatic transfer system was used to transfer the 50 mg 235 U samples from the irradiation position near the Godiva assembly to a remote shielded counting room containing the NE 213 spectrometer and associated electronics. Data were acquired in sixty-four 0.5 s time bins and over an energy range 1 to 7 MeV. Comparisons between these measurements and a detailed model calculation performed at Los Alamos is presented
Investigation of short-living fission products from the spontaneous fission of Cf-252
International Nuclear Information System (INIS)
Klonk, H.
1976-01-01
In this paper, a method of separating and measuring fission products of Cf-252 is presented. The measurement was achieved by means of γ-spectrometry and thus provides a quantitative analysis with a good separation of the fission products with respect to both atomic number Z and mass number A. The separation of the fission products from the fission source was achieved by means of solid traps. An automatic changing apparatus made it possible to keep irradiation and measuring times short, so even very short-lived fission products could be registered. The quantitative evaluation of primary fission products was made possible by correction according to Bateman equations. With that, the yields of single nuclides and the dispersion of charge can be determined. (orig./WL) [de
Neutron dosimetry for radiation damage in fission and fusion reactors
International Nuclear Information System (INIS)
Smith, D.L.
1979-01-01
The properties of materials subjected to the intense neutron radiation fields characteristic of fission power reactors or proposed fusion energy devices is a field of extensive current research. These investigations seek important information relevant to the safety and economics of nuclear energy. In high-level radiation environments, neutron metrology is accomplished predominantly with passive techniques which require detailed knowledge about many nuclear reactions. The quality of neutron dosimetry has increased noticeably during the past decade owing to the availability of new data and evaluations for both integral and differential cross sections, better quantitative understanding of radioactive decay processes, improvements in radiation detection technology, and the development of reliable spectrum unfolding procedures. However, there are problems caused by the persistence of serious integral-differential discrepancies for several important reactions. There is a need to further develop the data base for exothermic and low-threshold reactions needed in thermal and fast-fission dosimetry, and for high-threshold reactions needed in fusion-energy dosimetry. The unsatisfied data requirements for fission reactor dosimetry appear to be relatively modest and well defined, while the needs for fusion are extensive and less well defined because of the immature state of fusion technology. These various data requirements are examined with the goal of providing suggestions for continued dosimetry-related nuclear data research
International Nuclear Information System (INIS)
Damm, G.; Thiel, K.
1977-01-01
The age determined by counting fission tracks of lunar and meteorite materials is obviously falsified by additional fission track parts not to be accounted for by the spontaneous fission of uranium 238. For this p and n induced fissions of U, Th and other hreavy elements through the cosmic radiation come into consideration. In order to determine the possible part of such interference factors, a simulation experiment at the proton synchrocycloton (CERN, Geneva) has been carried out and independently of this, the production rates for the p and n induced U, Th, Bi, Pb and Au in the surface-near regolith layers of the moon were calculated. It could be seen that the irradiation age as well as the spacial distribution of the heavy metals in the samples to be dated must be considered. (RB) [de
Measurements of fission cross-sections and of neutron production rates
International Nuclear Information System (INIS)
Billaud, P.; Clair, C.; Gaudin, M.; Genin, R.; Joly, R.; Leroy, J.L.; Michaudon, A.; Ouvry, J.; Signarbieux, C.; Vendryes, G.
1958-01-01
a) Measurements of neutron induced fission cross-sections in the low energy region. The variation of the fission cross sections of several fissile isotopes has been measured and analysed, for neutron energies below 0,025 eV. The monochromator was a crystal spectrometer used in conjunction with a mechanical velocity selector removing higher order Bragg reflections. The fissile material was laid down on the plates of a fission chamber by painting technic. An ionization chamber, having its plates coated with thin 10 B layers, was used as the neutron flux monitor. b) Measurement of the fission cross section of 235 U. We intend to measure the variation of the neutron induced fission cross section of 235 U over the neutron energy range from 1 keV by the time of flight method. The neutron source is the uranium target of a pulsed 28 MeV electron linear accelerator. The detector is a large fission chamber, with parallel plates, containing about 10 g of 235 U (20 deposits of 25 cm diameter). The relative fission data were corrected for the neutron spectrum measured with a set of BF 3 proportional counters. c) Mean number ν of neutrons emitted in neutron induced fission. We measured the value of ν for several fissile isotopes in the case of fission induced by 14 MeV neutrons. The 14 MeV neutrons were produced by D (t, n) α reaction by means of a 300 kV Cockcroft Walton generator. (author) [fr
International Nuclear Information System (INIS)
Selby, H.D.; Mac Innes, M.R.; Barr, D.W.; Keksis, A.L.; Meade, R.A.; Burns, C.J.; Chadwick, M.B.; Wallstrom, T.C.
2010-01-01
We describe measurements of fission product data at Los Alamos that are important for determining the number of fissions that have occurred when neutrons are incident on plutonium and uranium isotopes. The fission-spectrum measurements were made using a fission chamber designed by the National Institute for Standards and Technology (NIST) in the BIG TEN critical assembly, as part of the Inter-laboratory Liquid Metal Fast Breeder Reactor (LMFBR) Reaction Rate (ILRR) collaboration. The thermal measurements were made at Los Alamos' Omega West Reactor. A related set of measurements were made of fission-product ratios (so-called R-values) in neutron environments provided by a number of Los Alamos critical assemblies that range from having average energies causing fission of 400-600 keV (BIG TEN and the outer regions of the Flattop-25 assembly) to higher energies (1.4-1.9 MeV) in the Jezebel, and in the central regions of the Flattop-25 and Flattop-Pu, critical assemblies. From these data we determine ratios of fission product yields in different fuel and neutron environments (Q-values) and fission product yields in fission spectrum neutron environments for 99 Mo, 95 Zr, 137 Cs, 140 Ba, 141,143 Ce, and 147 Nd. Modest incident-energy dependence exists for the 147 Nd fission product yield; this is discussed in the context of models for fission that include thermal and dynamical effects. The fission product data agree with measurements by Maeck and other authors using mass-spectrometry methods, and with the ILRR collaboration results that used gamma spectroscopy for quantifying fission products. We note that the measurements also contradict earlier 1950s historical Los Alamos estimates by ∼5-7%, most likely owing to self-shielding corrections not made in the early thermal measurements. Our experimental results provide a confirmation of the England-Rider ENDF/B-VI evaluated fission-spectrum fission product yields that were carried over to the ENDF/B-VII.0 library, except
Systematic evaluation of prompt neutron spectra in fission
International Nuclear Information System (INIS)
Osawa, Takaaki
1995-01-01
To create the nuclear data fail JEND-32, the prompt fission neutron spectra X(E) of 233 U, 235 U, 238 U and 239 Pu were reevaluated and some improvement were added to the calculation models. We tried to extend the calculation method of fission spectra of nuclides with poor measurement data in consideration of increasing the importance of nuclear data of minor actinoids. We improved and extended the following five points. (1) On JENDL-3.1, the fission spectra of principal fissible materials had been calculated by the Modland-Nix model which the neutron emissions of fragments were calculated under the approximation of the constant inverse process cross section. In the paper, the spectra were calculated by the use of the inverse process cross section depend on the energy obtained by the calculation of the optical model. The result showed the increase of low energy components and the softening effect of spectra (2) On JENDL-3.1, the all fission processes were assumed to undergo (n,f) reaction. In the paper, they were calculated by the multi-chance fission such as (n, n'f), (n, 2nf) and (n, 3nf) etc. Softening of the spectra (En > 6 MeV) was obtained by this method. (3) The level density parameter (LDP) has been assumed as a = A/C in either case of light fragment (LF) and heavy fragment (HF) in the original Madland-Nix model. But we used LDP based on the Ignatyuk model under consideration of the shell effects of nuclear fragments, hence the neutron spectra of heavy fragments were hardening. (4) Nuclear temperature of both fragments had been assumed to be the same at original model, but now R T = Tm/TmH was derived to calculate them. The ratio of middle/both side components of spectra was changed. (5) Unknown neutron fission spectra of minor actinide were able to the assumed on the basis of Moriyama-Ohnishi model. (S.Y.)
Proposal to represent neutron absorption by fission products by a single pseudo-fragment
International Nuclear Information System (INIS)
Tsibulya, A.M.; Kochetkov, A.L.; Kravchenko, I.V.; Nikolaev, M.N.
1991-01-01
The concentration of fission products during reactor operation is analyzed. The dependence of a composite fission product capture cross-section as a function of time and on the nature of the A of the fissile nuclide are investigated, and the neutron radiative capture in fission products of a thermal reactor is evaluated. It is concluded that neutron absorption by fission products can be described by pseudo-fragments. (author). 18 refs, 2 figs, 3 tabs
International Nuclear Information System (INIS)
Ruben, A.; Maerten, H.; Seeliger, D.
1990-01-01
A complex statistical theory of fission neutron emission combined with a phenomenological fission model has been used to calculate fission neutron data for 238 U. Obtained neutron multiplicities and energy spectra as well as average fragment energies for incidence energies from threshold to 20 MeV (including multiple-chance fission) are compared with traditional data representations. (author). 19 refs, 6 figs
International Nuclear Information System (INIS)
Barabanov, A.L.; Grechukhin, D.P.
1985-01-01
General analysis is conducted, and formulae for fission cross section and angular distribution of fission fragments of oriented nuclei by fast neutrons are presented. Geometrical coefficients making up the formulae permitting to carry out calculations for target nuclei with spins I=3/2, 5/2, 7/2 at interaction energies epsilon < or approximately 1 MeV are tabulated. Results of demonstrative calculation of fission fragment angular distribution of oriented sup(235)U nuclei by 0.1 <= epsilon <= 1.0 MeV neutrons reveal that angular distribution weakly depends on the set of permeability factors of neutron waves applied in the calculations
International Nuclear Information System (INIS)
Reber, E.L.; Gehrke, R.J.; Aryaeinejad, R.; Hartwell, J.K.
2005-01-01
Gamma-ray spectrometry measurements have been made of the fission yields of selected γ -rays emitted by the spontaneously fissioning isotopes 252 Cf and 244 Cm. The measured γ-rays were selected based on their relative abundance in the spectrum and their freedom from interference or, in a few instances, ease of interference correction. From these data and the cumulative and independent yield data of England and Rider, those γ-rays that are primarily produced by radioactive decay, as opposed to direct yield, were converted into the decays per spontaneous fission expressed in percent and compared to cumulative yield values of England and Rider. For those γ-rays whose production is dominated by direct (independent) yield, the ratio of γ-rays per spontaneous fission is reported. The γ-ray yield can be compared to the independent yield values of England and Rider when 100% of the direct feeding passes through the γ-ray. In those cases where both cumulative and independent yields contribute to the observed γ-ray emission rate, a direct comparison is not possible but a method to quantify the contribution from each is proposed. (author)
Above-threshold structure in {sup 244}Cm neutron-induced fission cross section
Energy Technology Data Exchange (ETDEWEB)
Maslov, V.M. [Radiation Physics and Chemistry Problems Inst., Minsk-Sosny (Belarus)
1997-03-01
The quasi-resonance structure appearing above the fission threshold in neutron-induced fission cross section of {sup 244}Cm(n,f) is interpreted. It is shown to be due to excitation of few-quasiparticle states in fissioning {sup 245}Cm and residual {sup 244}Cm nuclides. The estimate of quasiparticle excitation thresholds in fissioning nuclide {sup 245}Cm is consistent with pairing gap and fission barrier parameters. (author)
Prompt fission neutron spectra and anti νp
International Nuclear Information System (INIS)
Madland, D.G.
Methods used to obtain the evaluated prompt fisson neutron spectrum N(E) and the average prompt neutron multiplicity anti ν/sub p/ are reviewed. The relative influence of experimental data; interpolated, extrapolated, and fitted experimental data; systematics; and nuclear theory are considered for the cases where (a) abundant experimental data exist, (b) some experimental data exist, and (c) no experimental data exist. The Maxwellian and Watt distributions, and the determination of the parameters of these distributions by data fitting, are described and compared to recent new theoretical work on the calculation of N(E). Similarly, various expressions for anti γ/sub p/ that have been obtained by data fitting and systematics are described and compared to recent new theoretical work. Complications in the evaluation of N(E) and anti γ/sub p/ due to the onset of multiple-chance fission and the interrelationships between N(E), anti γΔ/sub p/ and the multiple-chance fission cross section are discussed using the example of the fission of 235 U. Some statistics and comments are given on the evaluations of N(E) and anti γ/sub p/ contained in ENDF/B-V, and a number of concluding recommendations are made for future evaluation work
Fission barriers of two odd-neutron heavy nuclei
International Nuclear Information System (INIS)
Koh, Meng-Hock; Bonneau, L.; Nhan Hao, T. V.; Duc, Dao Duy; Quentin, P.
2015-01-01
The fission barriers of two odd-neutron heavy odd nuclei,namely the 235 U and 239 Pu isotopes have been calculated within a self-consistent Hartree-Fock-plus-BCS approach with blocking. A Skyrme nucleon-nucleon effective interaction has been used together with a seniority force to describe pairing correlations. A full account of the genuine time-reversal symmetry breaking due to the presence of an unpaired nucleon has been incorporated at the mean field level. The SIII and SkM* parametrizations of the Skyrme interaction have been retained as well as for a part a newer parametrization, SLy5*. The seniority force parameters have been fitted to reproduce experimental odd-even mass differences in the actinide region. To assess the relevance of our calculated fission barrier distribution (as a function of the quantum numbers), we have studied the quality of our results with respect to the spectroscopy of band heads (for configurations deemed to be a pure single particle character) in the ground and fission isomeric states. Fission barriers of the considered odd nuclei have been compared with what is obtained for their even-even neighbouring isotopes (namely 234 U and 236 U, 238 Pu and 240 Pu respectively) to determine the so-called specialization energies. Various corrections and associated uncertainties have been discussed in order to compare our results with available data
Angular distributions in the neutron-induced fission of actinides
In 2003 the n_TOF Collaboration performed the fission cross section measurement of several actinides ($^{232}$Th, $^{233}$U, $^{234}$U, $^{237}$Np) at the n_TOF facility using an experImental setup made of Parallel Plate Avalanche Counters (PPAC). The method based on the detection of the 2 fragments in coincidence allowed to clearly disentangle the fission reactions among other types of reactions occurring in the spallation domain. We have been therefore able to cover the very broad neutron energy range 1eV-1GeV, taking full benefit of the unique characteristics of the n_TOF facility. Figure 1 shows an example obtained in the case of $^{237}$Np where the n_ TOF measurement showed that the cross section was underestimated by a large factor in the resonance region.
International Nuclear Information System (INIS)
Jin Jing; Wei Biao; Feng Peng; Tang Yuelin; Zhou Mi
2010-01-01
Based on the interdependent relationship between fission neutrons ( 252 Cf) and fission chain ( 235 U system), the paper presents the time-frequency feature analysis and recognition in fission neutron signal based on support vector machine (SVM) through the analysis on signal characteristics and the measuring principle of the 252 Cf fission neutron signal. The time-frequency characteristics and energy features of the fission neutron signal are extracted by using wavelet decomposition and de-noising wavelet packet decomposition, and then applied to training and classification by means of support vector machine based on statistical learning theory. The results show that, it is effective to obtain features of nuclear signal via wavelet decomposition and de-noising wavelet packet decomposition, and the latter can reflect the internal characteristics of the fission neutron system better. With the training accomplished, the SVM classifier achieves an accuracy rate above 70%, overcoming the lack of training samples, and verifying the effectiveness of the algorithm. (authors)
Absolute measurement of thermal neutron fluence and its application for fission track dating
International Nuclear Information System (INIS)
Ganzawa, Yoshihiro; Honda, Teruyuki; Nozaki, Tetsuya.
1988-01-01
The absolute measurements of thermal neutron fluence for fission track dating have been developed after the proceeding results of Honda et al. (1987). The 2,200 m/sec activation cross section of 197 Au (98.8 barn) is corrected to 87.4 barn (σa) by the three factors of the neutron temperature, Maxwellian distribution of thermal neutrons and non 1/v correction factor for the above absolute measurement. The calibrated factor (B th ) of standard glasses (SRM613, SRM962a, CN-1 and CN-2) and zeta-a (ζa) values for fission track dating are determined on the basis of these experimental results. The values of B th , (7.47 ± 0.29) x 10 9 for SRM613, (7.43 ± 0.34) x 10 9 for SRM962a, (2.50 ± 0.06) x 10 9 for CN-1 and (2.74 ± 0.06) x 10 9 for CN-2 closely agree with those reported previously by Honda et al. (1987). Further, the ζa values of 392.3 ± 16.5 for SRM962a and SRM613, 131.4 ± 3.1 for CN-1 and 144.1 ± 3.3 for CN-2 calculated from B th , effective thermal neutron fission cross-section σf (497.4 barn), isotopic abundance ratio 235 U/ 239 U, I (7.2527 x 10 -3 ) and spontaneous fission decay constant of 238 U, λ f (6.85 x 10 -17 a -7 ) show close agreement with ζ b values (392.5 ± 10.0, 131.6 ± 3.3, 140.1 ± 3.5) derived from the absolute age of Fish Canyon Tuff (27.9 ± 0.7 Ma) respectively. The fission track dating of zircons separated from Oligocene-Miocene tuff distributed in Eastern Hokkaido have been carried out by the external detector method using ζ a . The obtained ages are 28.6 ± 0.7 Ma (1 - 2) and 23.3 ± 0.7 Ma (3 - 2). These results agree well with the geologic age supported from Ashoro Fossil Fauna, K-Ar ages of volcanic rocks and stratigraphy in this area. (author)
Search for spontaneous fission activity in Salton Sea and Atlantis II hot brines
International Nuclear Information System (INIS)
Ter-Akopian, G.M.; Sokol, E.A.; Fam Ngoc Chuong; Ivanov, M.P.; Popeko, G.S.; Molzahn, D.; Lund, T.; Feige, G.; Brandt, R.
1984-01-01
A search for an unknown spontaneously fissioning activity, possibly due to SHE, was carried out with the Dubna 3 He-counter system. In the investigation of Salton Sea samples and Atlantis II samples no such activity could be detected with limits -12 g/g. (orig.)
Review of the neutron capture process in fission reactors
International Nuclear Information System (INIS)
Poenitz, W.P.
1981-07-01
The importance of the neutron capture process and the status of the more important cross section data are reviewed. The capture in fertile and fissile nuclei is considered. For thermal reactors the thermal to epithermal capture ratio for 238 U and 232 Th remains a problem though some improvements were made with more recent measurements. The capture cross section of 238 U in the fast energy range remains quite uncertain and a long standing discrepancy for the calculated versus experimental central reaction rate ratio C28/F49 persists. Capture in structural materials, fission product nuclei and the higher actinides is also considered
distributions for the thermal neutron induced fission of 234U
Directory of Open Access Journals (Sweden)
Al-Adili A.
2016-01-01
In addition, the analysis of thermal neutron induced fission of 234U(n,f will be discussed. Currently analysis of data is ongoing, originally taken at the ILL reactor. The experiment is of particular interest since no measurement exist of the mass and energy distributions for this system at thermal energies. One main problem encountered during analysis was the huge background of 235U(nth,f. Despite the negligible isotopic traces in the sample, the cross section difference is enormous. Solution to this parasitic background will be highlighted.
International Nuclear Information System (INIS)
Shmid, M.
1979-08-01
The main purpose of this work was to measure independent yields, in the thermal neutron fission of 235 U, of fission products which lie far from the centers of the isotopic and isobaric yield distributions. These measurements were used to test the predictions of semi-empirical systematics of fission yields and theoretical fission models. Delay times were measured as a function of temperature in the range 1200-2000degC. The very low delay times achieved in the present work permitted expanding the measurable region to the isotopes 147 , 148 Cs and 99 Rb which are of special interest in the present work. The delay times of Sr and Ba isotopes achieved were more than two orders of magnitude lower than values reported in the literature and thus short-lived isotopes of these elements could be separated for the first time by mass spectrometry. The half-lives of 147 Ba, 148 Ba, 149 La and 149 Ce were measured for the first time. The isotopic distributions of fission yields were measured for the elements Rb, Sr, Cs and Ba in the thermal neutron fission of 235 U, those of 99 Rb, 147 Cs and 148 Cs having been measured for the first time. A comparison of the experimental yields with the predictions of the currently accepted semi-empirical systematics of fission yields, which is the odd-even effect systematics, shows that the systematics succeeds in accounting for the strong odd-even proton effect and the weaker odd-even neutron effect and also in predicting the shape of the distributions in the central region. It is shown that prompt neutron emission broadens the distribution only slightly in the wing of heavy isotopes and more significantly in the wing of light isotopes. But the effect of prompt neutron emission cannot explain the large discrepancies existing between the predictions of fission models and the experimentally measured fission yield in the wings of the isotopic distributions. (B.G.)
Pomorski, K.; Nerlo-Pomorska, B.; Bartel, J.; Schmitt, C.
2018-03-01
The fission-fragment mass and total kinetic energy (TKE) distributions are evaluated in a quantum mechanical framework using elongation, mass asymmetry, neck degree of freedom as the relevant collective parameters in the Fourier shape parametrization recently developed by us. The potential energy surfaces (PES) are calculated within the macroscopic-microscopic model based on the Lublin-Strasbourg Drop (LSD), the Yukawa-folded (YF) single-particle potential and a monopole pairing force. The PES are presented and analysed in detail for even-even Plutonium isotopes with A = 236-246. They reveal deep asymmetric valleys. The fission-fragment mass and TKE distributions are obtained from the ground state of a collective Hamiltonian computed within the Born-Oppenheimer approximation, in the WKB approach by introducing a neck-dependent fission probability. The calculated mass and total kinetic energy distributions are found in good agreement with the data.
A comparison of microstructures in copper irradiated with fission, fusion, and spallation neutrons
International Nuclear Information System (INIS)
Muroga, T.; Heinisch, H.L.; Sommer, W.F.; Ferguson, P.D.
1992-01-01
The objective of this work is to investigate the effects of the neutron energy spectrum in low dose irradiations on the microstructure and mechanical properties of metals. The microstructures of pure copper irradiated to low doses at 36-90 C with spallation neutrons, fusion neutrons and fission neutrons are compared. The defect cluster densities for the spallation and fusion neutrons are very similar when compared on the basis of displacements per atom (dpa). In both cases, the density increases in proportion to the square root of the dpa. The difference in defect density between fusion neutrons and fission neutrons corresponds with differences observed in data on yield stress changes
International Nuclear Information System (INIS)
Piksaikin, V.M.; Isaev, S.G.; Goverdovski, A.A.; Pshakin, G.M.
1998-10-01
The document includes the following two reports: 'Correlation properties of delayed neutrons from fast neutron induced fission' and 'Method and set-up for measurements of trace level content of heavy fissionable elements based on delayed neutron counting. A separate abstract was prepared for each report
Energy Technology Data Exchange (ETDEWEB)
Koegler, Toni Joerg
2016-04-26
Neutron induced fission cross sections of actinides like the Pu-isotopes are of relevance for the development of nuclear transmutation technologies. For {sup 242}Pu, current uncertainties are of around 21%. Sensitivity studies show that the total uncertainty has to be reduced to below 5% to allow for reliable neutron physics simulations. This challenging task was performed at the neutron time-of-flight facility of the new German National Center for High Power Radiation Sources at HZDR, Dresden. Within the TRAKULA project, thin, large and homogeneous deposits of {sup 235}U and {sup 242}Pu have been produced successfully. Using two consecutively placed fission chambers allowed the determination of the neutron induced fission cross section of {sup 242}Pu relative to {sup 235}U. The areal density of the Plutonium targets was calculated using the measured spontaneous fission rate. Experimental results of the fast neutron induced fission of {sup 242}Pu acquired at nELBE will be presented and compared to recent experiments and evaluated data. Corrections addressing the neutron scattering are discussed by using results of different neutron transport simulations (Geant 4, MCNP 6 and FLUKA).
Evaluation of fission product neutron cross sections for JENDL
International Nuclear Information System (INIS)
1984-01-01
The recent activities on the evaluation of fission product (FP) neutron cross sections for JENDL (Japanese Evaluated Nuclear Data Library) are presented briefly. The integral test of JENDL-1 FP cross section file was performed using the CFRMF sample activation data and the STEK sample reactivity data, and the ratio of experiment to calculation was nearly constant for all the samples in the STEK measurement. Therefore, a tentative analysis was performed by applying the correction to the calculated scattering reactivity component. Better agreement with the experiment was obtained after applying this correction in most cases. The evaluation work on the JENDL-2 FP neutron cross sections is now in progress. The improvement of the data evaluation is presented in an itemized form. The JENDL-2 FP file will contain the evaluated data for 100 nuclides from Kr to Tb. The improvement and the future scope of the integral test for JENDL-2 FP data are summarized. (Asami, T.)
Fission neutron damage rates and efficiencies in several metals
International Nuclear Information System (INIS)
Klabunde, C.E.; Coltman, R.R. Jr.
1981-11-01
Initial rates of resistivity-measured low-temperature damage production by fission-spectrum fast neutrons have been determined for 14 metals in the same very well characterized irradiation facility. Six of these metals were fcc, 5 bcc, and 3 hcp. Most were of quite high purity. Observed damage rates, after correction for all known extraneous resistivity-producing effects, were compared with rates predicted by the damage calculation code RECOIL, using parameters chosen from the literature. These parameters, effective displacement threshold energy, E/sub d/, and Frenkel-pair resistivity, rho/sub F/, were in many cases only best estimates, the further refinement of which may be aided by the present results. Damage efficiencies (measured/predicted rates) follow the same trends by crystal classes as seen in other fast-neutron studies
Gamma ray transitions in de-excitation of 252Cf spontaneous fission fragments
International Nuclear Information System (INIS)
Khan, N.A.; Rashid, K.; Ahmad, M.; Qureshi, I.E.; Alam, G.D.; Ali, A.; Bhatti, N.; Horsch, F.
1983-11-01
Gamma rays in the range from 60 keV to 730 keV have been observed following the spontaneous fission of 252 Cf, with high resolution Ge(Li) detector, full width at half maximum (FWHM) of 700 eV at 122 keV, in coincidence with the two fission fragments observed with surface barrier detectors. A total number of 18, 636, 549 events were recorded over a run period of about 150 hours stretching over three weeks. The events were sorted to generate gamma ray spectra belonging to 2 amu intervals gamma of the fragment masses and 6 MeV intervals of the total kinetic energy released. Some of the prominent gamma lines belonging to various masses of the fission fragments have been identified. For some gamma lines, the intensities have been evaluated as a function of the total kinetic energy of the fission fragments. (authors)
The universal library of fission products and delayed neutron group yields
International Nuclear Information System (INIS)
Koldobskiy, A.B.; Zhivun, V.M.
1997-01-01
A new fission product yield library based on the Semiempirical method for the estimation of their mass and charge distribution is described. Contrary to other compilations, this library can be used with all possible excitation energies of fissionable actinides. The library of delayed neutron group yields, based on the fission product yield compilation, is described as well. (author). 15 refs, 4 tabs
Study of scission shapes in spontaneous ternary fission of 252Cf
International Nuclear Information System (INIS)
Singer, P.; Schwalm, D.; Thirolf, P.; Goennenwein, F.; Hesse, M.
1995-06-01
A new kinematic study on the ternary fission of 252 Cf has been conducted by registering prompt neutrons and fission γ rays coincidence with light charged particles (LCP) and fission fragments. The aim is to investigate changes in fragment deformation energy between the binary and ternary fission modes from measured prompt neutron angular distributions and multiplicities, and to explore the influence of light particle emission on the energy distribution, multiplicity and angular anisotropy of γ rays emitted during fragment de-excitation. The experiment was performed at the MPI Heidelberg using the Darmstadt-Heidelberg crystal ball spectrometer as γ-ray and neutron detector. Fragments were identified by a double-E measurement with an angular sensitive twin ionization chamber (IC). Light charged particles from fission were measured by ΔE-E telescopes composed of ΔE ICs and silicon PIN diodes. The telescopes enable to identify various LCPs which are emitted much more rarely than ternary α particles. The parameters of the experiment and the method of data analysis are described and first results presented. (orig.)
Fission fragment simulation of fusion neutron radiation effects on bulk mechanical properties
International Nuclear Information System (INIS)
Van Konynenburg, R.A.; Mitchell, J.B.; Guinan, M.W.; Stuart, R.N.; Borg, R.J.
1976-01-01
This research demonstrates the feasibility of using homogeneously-generated fission fragments to simulate high-fluence fusion neutron damage in niobium tensile specimens. This technique makes it possible to measure radiation effects on bulk mechanical properties at high damage states, using conveniently short irradiation times. The primary knock-on spectrum for a fusion reactor is very similar to that produced by fission fragments, and nearly the same ratio of gas atoms to displaced atoms is produced in niobium. The damage from fission fragments is compared to that from fusion neutrons and fission reactor neutrons in terms of experimentally measured yield strength increase, transmission electron microscopy (TEM) observations, and calculated damage energies
International Nuclear Information System (INIS)
Kobayashi, Katsuhei; Kobayashi, Tooru
1992-01-01
The 235 U fission spectrum-averaged cross sections for 13 threshold reactions were measured with the fission plate (27 cm in diameter and 1.1 cm thick) at the heavy water thermal neutron facility of the Kyoto University Reactor. The Monte Carlo code MCNP was applied to check the deviation from the 235 U fission neutron spectrum due to the room-scattered neutrons, and it was found that the resultant spectrum was close to that of 235 U fission neutrons. Supplementally, the relations to derive the absorbed dose rates with the fission plate were also given using the calculated neutron spectra and the neutron Kerma factors. Finally, the present values of the fission spectrum-averaged cross sections were employed to adjust the 235 U fission neutron spectrum with the NEUPAC code. The adjusted spectrum showed a good agreement with the Watt-type fission neutron spectrum. (author)
Dispersion of the Neutron Emission in U{sup 235} Fission
Feynman, R. P.; de Hoffmann, F.; Serber, R.
1955-01-01
Equations are developed which allow the calculation of the average number of neutrons per U{sup235} fission from experimental measurements. Experimental methods are described, the results of which give a value of (7.8 + 0.6){sup ½} neutrons per U{sup 235} thermal fission.
International Nuclear Information System (INIS)
Capote Noy, R.
2013-09-01
A summary is given of the Second Research Coordination Meeting on Prompt Fission Neutron Spectra of Actinides. Experimental data and modelling methods on prompt fission neutron spectra were reviewed. Extensive technical discussions held on theoretical methods to calculate prompt fission spectra. Detailed coordinated research proposals have been agreed. Summary reports of selected technical presentations at the meeting are given. The resulting work plan of the Coordinated Research Programme is summarized, along with actions and deadlines. (author)
Induction of chromosomal aberrations in human lymphocytes by fission neutrons
International Nuclear Information System (INIS)
Silva, Marcia Augusta da; Coelho, Paulo Rogerio Pinto; Bartolini, Paolo; Okazaki, Kayo
2009-01-01
Chromosome aberrations induced by sparsely ionizing radiation (low-LET) are well known and cytogenetic analyses of irradiated human lymphocytes have been widely applied to biological dosimetry. However, much less is known about chromosome aberrations induced by densely ionizing radiation (high LET), such as that of alpha particles or neutrons. Such particles induce DNA strand breaks, as well as chromosome breakage and rearrangements of high complexity. This damage is more localized and less efficiently repaired than after X- or γ-ray irradiation. This preferential production of complex aberrations by densely ionizing radiation is related to the unique energy deposition patterns, which produces highly localized multiple DNA damage at the chromosomal level. A better knowledge of the interactions between different types of radiation and cellular DNA is of importance, not only from the radiobiological viewpoint but also for dosimetric and therapeutic purposes. The objective of the present study was to analyse the cytogenetic effects of fission neutrons on peripheral blood lymphocytes in order to evaluate structural and numerical aberrations and number of cells in the different mitotic cycles. So, blood samples from five healthy donors, 22-25 years old, of both sexes, were irradiated in the Research Reactor IEA-R1 of our Institute (IPEN/CNEN-SP) with thermal and fast neutrons at doses of 0.2; 0.3; 0.5 and 1.0 Gy. The γ contribution to the total absorbed dose was about 30%. These doses were monitored by thermoluminescent dosemeters: LiF-600 (for neutrons) and LiF-700 (for γ-rays). The data concerning structural aberrations were evaluated with regard to three parameters: percentage of cells with aberrations, number of aberrations/cell and number of dicentric/cell. The cytogenetic results showed an increase in the three parameters after irradiation with neutrons, as a function of radiation dose. Apparently, there was no influence of neutrons on the kinetics of cellular
Neutron emission in fission of highly excited californium nuclei (E* = 76 MeV)
International Nuclear Information System (INIS)
Blinov, M.V.; Bordyug, V.M.; Kozulin, E.M.; Levitovich, M.; Mozhaev, A.N.; Muzychka, Yu.A.; Penionzhkevich, Yu.E.; Pustyl'nik, B.I.
1990-01-01
Differential cross sections for neutron production have been measured in fission of excited californium nuclei produced in the reaction 238 U + 12 C (105 MeV). It follows from analysis of the experimental results that the number of neutrons emitted before fission considerably exceeds the number obtained in the framework of the standard statistical model. On the basis of the multiplicity of neutrons they authors have estimated the time of fission of the excited nucleus. The dependence of the number of neutrons and their average energies on the mass of the fragments is determined
The 235U prompt fission neutron spectrum measured by the Chi-Nu project at LANSCE
Directory of Open Access Journals (Sweden)
Gomez J.A.
2017-01-01
Full Text Available The Chi-Nu experiment aims to accurately measure the prompt fission neutron spectrum for the major actinides. At the Los Alamos Neutron Science Center (LANSCE, fission can be induced with neutrons ranging from 0.7 MeV and above. Using a two arm time-of-flight (TOF technique, the fission neutrons are measured in one of two arrays: a 22-6Li glass array for lower energies, or a 54-liquid scintillator array for outgoing energies of 0.5 MeV and greater. Presented here are the collaboration's preliminary efforts at measuring the 235U PFNS.
Energy Technology Data Exchange (ETDEWEB)
Gautherin, C.; Houry, M.; Korten, W.; Le Coz, Y.; Lucas, R.; Thiesen, Ch. [Dept. d`Astrophysique, de la Physique des Particules, de la Physique Nucleaire et de l`Instrumentation Associee, CEA Centre d`Etudes de Saclay, 91 - Gif-sur-Yvette (France); Badimon, C.; Barreau, G.; Doan, T.P.; Pedemay, G. [Centre d`Etudes Nucleaires, Bordeaux-1 Univ., 33 Gradignan (France); Belier, G.; Girod, M.; Meot, M.V. [CEA Centre d`Etudes de Bruyeres-le-Chatel, 91 (France); Astier, G.; Meot, V.; Peru, S. [CEA Centre d`Etudes de Bruyeres-le-Chatel, 91 (France); Astier, A.; Ducroux, L.; Meyer, M.; Redon, N. [Inst.de Physique Nucleaire, Lyon-1 Univ., 69 - Villeurbanne (France)
1997-06-01
Isomeric states have been studied in fission fragments produced by spontaneous fission of {sup 252}Cf. 34 isomeric nuclei have been identified by using coincidences between {gamma}-rays detected in EUROGAM II and fission fragments detected in photovoltaic cells. Lifetimes from 20 ns up to 2 {mu}s have been measured. Microscopic interpretation of the isomeric levels discovered has been tried by means of the Hartree-Fock-Bogolyubov procedure using Gogny force. It was found that the {sup 152,154,156}Nd nuclei have prolate deformation in their ground state; the rotational band built on this ground state is well reproduced by the calculation. For these nuclei the 2 quasi-particle excited states energies are above 1 MeV in agreement with the experiment. The computation confirms the similitude of the {sup 156}Nd and {sup 158}Sm isomeric states associated to neutron 2 quasi-particles of J{sup {pi}} K{sup {pi}} = 5{sup -} ({nu} 5/2 (642) x {nu} 5/2 (523)) while such similitude does not occur for the isotone nuclei {sup 154}Nd and {sup 156}Sm. The computation predicts a proton 2 quasi-particle excited states of J{sup {pi}} = 5{sup -}, near the isomeric level measured in {sup 156}Sm but not for that of {sup 154}Nd. Concerning the {sup 152}Nd the calculated level density is very near that of the states measured in the 1.6 to 2.3 MeV interval. However, the lack of precise information on spins and parities of the measured levels does make not possible a confrontation with the calculations. An up-graded equipment implying 32 photovoltaic cells instead of 2 cells is to be developed and installed by the EUROGAM 3 refs.
Energy spectra of neutrons accompanying the emission fission of 238U
International Nuclear Information System (INIS)
Smirenkin, G.N.; Lovchikova, G.N.; Trufanov, A.M.; Svirin, M.I.; Polyakov, A.V.; Vinogradov, V.A.; Dmitriev, V.D.; Boykov, G.S.
1996-01-01
The spectra of fission neutrons emitted from 238U are measured for the first time by the time-of-flight method at incident-neutron energies of 16.0 and 17.7 MeV. Analysis of the neutron spectra shows that experimental results at incident-neutron energies of 14.7, 16.0, and 17.7 MeV (above the threshold of chance fission) differ significantly from those obtained at a neutron energy of 2.9 MeV (below the threshold of chance fission). Owing to the prefission emission of neutrons, the observed spectra of neutrons from emission fission exhibit a characteristic growth of the neutron yield in both hard and soft sections of the spectrum of secondary neutrons. This growth manifests itself as a step in the first case and as a rise in the second case, where it results in a noticeable excess of neutrons over the statistical-model predictions for E<2 MeV. The first feature in the spectra of neutrons from emission fission can be associated with the nonequilibrium decay of an excited fissile nucleus. On the contrary, the origin of the second feature has yet to be clarified. Additional measurements of angular distributions of secondary neutrons may prove helpful in this respect
Evaluation of Neutron Induced Reactions for 32 Fission Products
Energy Technology Data Exchange (ETDEWEB)
Kim, Hyeong Il
2007-02-15
Neutron cross sections for 32 fission products were evaluated in the neutron-incident energy range from 10{sup -5} eV to 20 MeV. The list of fission products consists of the priority materials for several applications, extended to cover complete isotopic chains for three elements. The full list includes 8 individual isotopes, {sup 95}Mo, {sup 101}Ru, {sup 103}Rh, {sup 105}Pd, {sup 109}Ag, {sup 131}Xe, {sup 133}Cs, {sup 141}Pr, and 24 isotopes in complete isotopic chains for Nd (8), Sm (9) and Dy (7). Our evaluation methodology covers both the low energy region and the fast neutron region.In the low energy region, our evaluations are based on the latest data published in the Atlas of Neutron Resonances. This resource was used to infer both the thermal values and the resolved resonance parameters that were validated against the capture resonance integrals. In the unresolved resonance region we performed the additional evaluation by using the averages of the resolved resonances and adjusting them to the experimental data.In the fast neutron region our evaluations are based on the nuclear reaction model code EMPIRE-2.19 validated against the experimental data. EMPIRE is the modular system of codes consisting of many nuclear reaction models, including the spherical and deformed Optical Model, Hauser-Feshbach theory with the width fluctuation correction and complete gamma-ray emission cascade, DWBA, Multi-step Direct and Multi-step Compound models, and several versions of the phenomenological preequilibrium models. The code is equipped with a power full GUI, allowing an easy access to support libraries such as RIPL and CSISRS, the graphical package, as well the utility codes for formatting and checking. In general, in our calculations we used the Reference Input Parameter Library, RIPL, for the initial set model parameters. These parameters were properly adjusted to reproduce the available experimental data taken from the CSISRS library. Our evaluations cover cross
Evaluation of Neutron Induced Reactions for 32 Fission Products
International Nuclear Information System (INIS)
Kim, Hyeong Il
2007-02-01
Neutron cross sections for 32 fission products were evaluated in the neutron-incident energy range from 10 -5 eV to 20 MeV. The list of fission products consists of the priority materials for several applications, extended to cover complete isotopic chains for three elements. The full list includes 8 individual isotopes, 95 Mo, 101 Ru, 103 Rh, 105 Pd, 109 Ag, 131 Xe, 133 Cs, 141 Pr, and 24 isotopes in complete isotopic chains for Nd (8), Sm (9) and Dy (7). Our evaluation methodology covers both the low energy region and the fast neutron region.In the low energy region, our evaluations are based on the latest data published in the Atlas of Neutron Resonances. This resource was used to infer both the thermal values and the resolved resonance parameters that were validated against the capture resonance integrals. In the unresolved resonance region we performed the additional evaluation by using the averages of the resolved resonances and adjusting them to the experimental data.In the fast neutron region our evaluations are based on the nuclear reaction model code EMPIRE-2.19 validated against the experimental data. EMPIRE is the modular system of codes consisting of many nuclear reaction models, including the spherical and deformed Optical Model, Hauser-Feshbach theory with the width fluctuation correction and complete gamma-ray emission cascade, DWBA, Multi-step Direct and Multi-step Compound models, and several versions of the phenomenological preequilibrium models. The code is equipped with a power full GUI, allowing an easy access to support libraries such as RIPL and CSISRS, the graphical package, as well the utility codes for formatting and checking. In general, in our calculations we used the Reference Input Parameter Library, RIPL, for the initial set model parameters. These parameters were properly adjusted to reproduce the available experimental data taken from the CSISRS library. Our evaluations cover cross sections for almost all reaction channels
He and Be ternary spontaneous fission of sup 2 sup 5 sup 2 Cf
Hwang, J K; Ramayya, A V; Hamilton, J H
2002-01-01
Ternary and binary fission studies of sup 2 sup 5 sup 2 Cf have been carried out by using the Gammasphere detector array with light charged particle (LCD) detectors. The relative sup 4 He and sup 5 He ternary fission yields were determined. The kinetic energies of the sup 5 He and sup 4 He ternary particles were found to be approximately 11 and 16 MeV, respectively. The sup 5 He particles contribute 10-20 % to the total observed alpha ternary yield. The data indicate that in nuclei with octupole deformations the population for the negative parity bands might be enhanced in the alpha ternary fission. >From LCP-gamma double gated spectra, neutron multiplicity distributions for alpha ternary fission pairs were measured. The average neutron multiplicity decreases about 0.7 AMU in going from the binary to alpha ternary fission in the approximately same mass splittings (104-146). From the analysis of the gamma-gamma matrix gated on the sup 1 sup 0 Be particles, the two fragment pairs of sup 1 sup 3 sup 8 Xe - sup 1...
Fission product yields from 6 to 9 MeV neutron induced fission of 235U and 238U
International Nuclear Information System (INIS)
Chapman, T.C.
1978-01-01
The yields of 28 mass chains have been measured for fission of 235 U and 238 U induced by neutrons at four different energies from 6.0 to 9.1 MeV. This is the first experimental measurement where sufficient energy resolution was obtained to observe the effect of the onset of second-chance fission in the case of symmetric fission. The 111 Ag results are compared with measurements at other neutron energies and with previous theoretical predictions. Several of the nuclide results are presented in graphical form, and all nuclide results are presented in tabular form, as a function of neutron energy. The mass chains measured range from 84 to 156, and their half-lives range from 18 minutes to 30 years
8-group relative delayed neutron yields for epithermal neutron induced fission of 235U and 239Pu
International Nuclear Information System (INIS)
Piksaikin, V.M.; Kazakov, L.E.; Isaev, S.G.; Korolev, G.G.; Roshchenko, V.A.; Tertychnyj, R.G
2002-01-01
An 8-group representation of relative delayed neutron yields was obtained for epithermal neutron induced fission of 235 U and 239 Pu. These data were compared with ENDF/B-VI data in terms of the average half- life of the delayed neutron precursors and on the basis of the dependence of reactivity on the asymptotic period. (author)
Energy Technology Data Exchange (ETDEWEB)
Casoli, P.; Authier, N. [CEA, Centre de Valduc, 21120 Is-sur-Tille (France); Laurec, J.; Bauge, E.; Granier, T. [CEA, Centre DIF, 91297 Arpajon (France)
2011-07-01
In the 1970's and early 1980's, an experimental program was performed on the facilities of the CEA Valduc Research Center to measure several actinide-fission product yields. Experiments were, in particular, completed on the Caliban and Prospero metallic core reactors to study fission-neutron-induced reactions on {sup 233}U, {sup 235}U, and {sup 239}Pu. Thick actinide samples were irradiated and the number of nuclei of each fission product was determined by gamma spectrometry. Fission chambers were irradiated simultaneously to measure the numbers of fissions in thin deposits of the same actinides. The masses of the thick samples and the thin deposits were determined by mass spectrometry and alpha spectrometry. The results of these experiments will be fully presented in this paper for the first time. A description of the Caliban and Prospero reactors, their characteristics and performances, and explanations about the experimental approach will also be given in the article. A recent work has been completed to analyze and reinterpret these measurements and particularly to evaluate the associated uncertainties. In this context, calculations have also been carried out with the Monte Carlo transport code Tripoli-4, using the published benchmarked Caliban description and a three-dimensional model of Prospero, to determine the average neutron energy causing fission. Simulation results will be discussed in this paper. Finally, new fission yield measurements will be proposed on Caliban and Prospero reactors to strengthen the results of the first experiments. (authors)
High-energy Neutron-induced Fission Cross Sections of Natural Lead and Bismuth-209
Tarrio, D; Carrapico, C; Eleftheriadis, C; Leeb, H; Calvino, F; Herrera-Martinez, A; Savvidis, I; Vlachoudis, V; Haas, B; Koehler, P; Vannini, G; Oshima, M; Le Naour, C; Gramegna, F; Wiescher, M; Pigni, M T; Audouin, L; Mengoni, A; Quesada, J; Becvar, F; Plag, R; Cennini, P; Mosconi, M; Rauscher, T; Couture, A; Capote, R; Sarchiapone, L; Vlastou, R; Domingo-Pardo, C; Dillmann, I; Pavlopoulos, P; Karamanis, D; Krticka, M; Jericha, E; Ferrari, A; Martinez, T; Trubert, D; Oberhummer, H; Karadimos, D; Plompen, A; Isaev, S; Terlizzi, R; Cortes, G; Cox, J; Cano-Ott, D; Pretel, C; Colonna, N; Berthoumieux, E; Vaz, P; Heil, M; Lopes, I; Lampoudis, C; Walter, S; Calviani, M; Gonzalez-Romero, E; Embid-Segura, M; Stephan, C; Igashira, M; Papachristodoulou, C; Aerts, G; Tavora, L; Berthier, B; Rudolf, G; Andrzejewski, J; Villamarin, D; Ferreira-Marques, R; Tain, J L; O'Brien, S; Reifarth, R; Kadi, Y; Neves, F; Poch, A; Kerveno, M; Rubbia, C; Lazano, M; Dahlfors, M; Wisshak, K; Salgado, J; Dridi, W; Ventura, A; Andriamonje, S; Assimakopoulos, P; Santos, C; Voss, F; Ferrant, L; Patronis, N; Chiaveri, E; Guerrero, C; Perrot, L; Vicente, M C; Lindote, A; Praena, J; Baumann, P; Kappeler, F; Rullhusen, P; Furman, W; David, S; Marrone, S; Tassan-Got, L; Gunsig, F; Alvarez-Velarde, F; Massimi, C; Mastinu, P; Pancin, J; Papadopoulos, C; Tagliente, G; Haight, R; Chepel, V; Kossionides, E; Badurek, G; Marganiec, J; Lukic, S; Pavlik, A; Goncalves, I; Duran, I; Alvarez, H; Abbondanno, U; Fujii, K; Milazzo, P M; Moreau, C
2011-01-01
The CERN Neutron Time-Of-Flight (n\\_TOF) facility is well suited to measure small neutron-induced fission cross sections, as those of subactinides. The cross section ratios of (nat)Pb and (209)Bi relative to (235)U and (238)U were measured using PPAC detectors. The fragment coincidence method allows to unambiguously identify the fission events. The present experiment provides the first results for neutron-induced fission up to 1 GeV for (nat)Pb and (209)Bi. A good agreement with previous experimental data below 200 MeV is shown. The comparison with proton-induced fission indicates that the limiting regime where neutron-induced and proton-induced fission reach equal cross section is close to 1 GeV.
Calculating the mass distribution of heavy nucleus fission product by neutrons
International Nuclear Information System (INIS)
Gudkov, A.N.; Koldobskij, A.B.; Kolobashkin, V.M.; Semenova, E.V.
1981-01-01
The technique of calculating the fission product mass yields by neutrons which are necessary for performing nucleus physical calculations in designing nuclear reactor cores is considered. The technique is based on the approximation of fission product mass distribution over the whole mass range by five Gauss functions. New analytical expressions for determining energy weights of used gaussians are proposed. The results of comparison of experimental data with calculated values for fission product mass obtained for reference processes in the capacity of which the fission reactions are chosen: 233 U, 235 U fission by thermal neutrons, 232 Th, 233 U, 235 U, 238 U by fission spectrum neutrons and 14 MeV neutrons and for 232 Th fission reactions by 11 MeV neutrons and 238 U by 7.7 MeV neutrons. On the basis of the analysis of results obtained the conclusion is drawn on a good agreement of fission product mass yield calculation values obtained using recommended values of mass distribution parameters with experimental data [ru
Observed mass distribution of spontaneous fission fragments from samples of lime - an SSNTD study
Paul, D; Ghose, D; Sastri, R C
1999-01-01
SSNTD is one of the most commonly used detectors in the studies involving nuclear phenomena. The ease of registration of the presence of alpha particles and fission fragments has made it particularly suitable in studies where stable long exposures are needed to extract reliable information. Studies on the presence of alpha emitting nuclides in the environment assume importance since they are found to be carcinogenic. Lime samples from Silchar in Assam of Eastern India have shown the presence of spontaneous fission fragments besides alphas. In the present study we look at the ratio of the average mass distribution of these fission fragments, that gives us an indication of the presence of the traces of transuranic elements.
Spontaneous-fission half-lives for even nuclei with Z> or =92
International Nuclear Information System (INIS)
Randrup, J.; Larsson, S.E.; Moller, P.; Nilsson, S.G.; Pomorski, K.; Sobiczewski, A.
1976-01-01
The spontaneous-fission process for doubly even nuclei with Z> or =92 is studied in a semiempirical WKB framework. One-dimensional fission barrier potentials are established from theoretical deformation-energy surfaces based on the droplet model and the modified-oscillator model. The effects of axial asymmetry as well as reflection asymmetry have been taken into account. Macroscopic (irrotational flow) inertial-mass functions and, alternatively, microscopic (cranking model) inertial mass parameters have been employed for the calculation of the fission half-lives. With one over-all normalization parameter it is possible to fit the experimental half-lives to within a factor of 20 on the average. The resulting effective inertial-mass functions are used to estimate the stability of the transactinide elements. Only minor differences with previous estimates for the r process and superheavy nuclei are encountered
Mechanism of fission of neutron-deficient actinoids nuclides
International Nuclear Information System (INIS)
Sueki, Keisuke; Nakahara, Hiromichi; Tanase, Masakazu; Nagame, Yuichiro; Shinohara, Nobuo; Tsukada, Kazuaki.
1996-01-01
A heavy ion reaction ( 19 F+ 209 Bi) is selected. The reaction produces neutron-deficient 228 U which is compound nucleus with a pair of Rb(z=37) and Cs(Z=55). Energy dissipation problem of nucleus was studied by measuring the isotope distribution of two fissile nuclides. Bismuth metal evaporated on aluminium foil was irradiated by 19 F with the incident energy of 105-128 MeV. We concluded from the results that the excess energy of reaction system obtained with increasing the incident energy is consumed by (1) light Rb much more than Cs and (2) about 60% of energy is given to two fission fragments and the rest 40% to the translational kinetic energy or unknown anomalous γ-ray irradiation. (S.Y.)
Fission-neutron displacement cross sections in metals
International Nuclear Information System (INIS)
Takamura, Saburo; Aruga, Takeo; Nakata, Kiyotomo
1985-01-01
The sensitivity damage rates for 22 metals were measured after fission-spectrum neutron irradiation at low temperature and the experimental damage rates were compared with the theoretical calculation. The relation between the theoretical displacement cross section and the atomic weight of metals can be written by two curves; one is for fcc and hcp metals, and another is for bcc metals. On the other hand, the experimental displacement cross section versus atomic weight is shown approximately by a curve for both fcc and bcc metals, and the cross section for hcp metals deviates from the curve. The defect production efficiency is 0.3-0.4 for fcc metals and 0.6-0.8 for bcc metals. (orig.)
Mechanism of fission of neutron-deficient actinoids nuclides
Energy Technology Data Exchange (ETDEWEB)
Sueki, Keisuke; Nakahara, Hiromichi [Tokyo Metropolitan Univ., Hachioji (Japan). Faculty of Science; Tanase, Masakazu; Nagame, Yuichiro; Shinohara, Nobuo; Tsukada, Kazuaki
1996-01-01
A heavy ion reaction ({sup 19}F+{sup 209}Bi) is selected. The reaction produces neutron-deficient {sup 228}U which is compound nucleus with a pair of Rb(z=37) and Cs(Z=55). Energy dissipation problem of nucleus was studied by measuring the isotope distribution of two fissile nuclides. Bismuth metal evaporated on aluminium foil was irradiated by {sup 19}F with the incident energy of 105-128 MeV. We concluded from the results that the excess energy of reaction system obtained with increasing the incident energy is consumed by (1) light Rb much more than Cs and (2) about 60% of energy is given to two fission fragments and the rest 40% to the translational kinetic energy or unknown anomalous {gamma}-ray irradiation. (S.Y.)
Extensions to COGEND for ENDF/B-V output of spontaneous fission decay data
International Nuclear Information System (INIS)
Tobias, A.
1978-06-01
The computer code COGEND, used to produce ENDF/B-IV or -V format nuclear decay scheme data, has been modified in order to extend its range of application. Details are given of the additional facilities which permit the handling of spontaneous fission decay data including any associated continuous spectra. In order to accommodate these additional features it is necessary to increase the core region by 4 kilobytes. (author)
Total and spontaneous fission half-lives of the americium and curium nuclides
International Nuclear Information System (INIS)
Holden, N.E.
1984-01-01
The total half-life and the half-life for spontaneous fission are evaluated for the various long-lived nuclides of interest. Recommended values are presented for 241 Am, /sup 242m/Am, 243 Am, 242 Cm, 243 Cm, 244 Cm, 245 Cm, 246 Cm, 247 Cm, 248 Cm, and 250 Cm. The uncertainties are provided at the 95% confidence limit for each of the recommended values
Fresnel zone plate imaging of a 252Cf spontaneous fission source
International Nuclear Information System (INIS)
Stalker, K.T.; Hessel, K.R.
1976-11-01
The feasibility of coded aperture imaging for nuclear fuel motion monitoring is shown using Cf 252 spontaneous fission source. The theory of coded aperture imaging for Fresnel zone plate apertures is presented and design considerations for zone plate construction are discussed. Actual images are obtained which demonstrate a transverse resolution of 1.7 mm and a tomographic resolution of 1.5 millimeters. The capability of obtaining images through 12.7 mm of stainless steel is also shown
Utilisation of prompt fission neutron technology in Greenfields uranium exploration
International Nuclear Information System (INIS)
Mutz, P.R.
2007-01-01
Conventionally, gamma detection technology has been used in uranium exploration programs for the initial detection of uranium as well as for a determination of uranium concentration. Geophysical logging companies use wireline gamma probes to measure uranium within boreholes, and field technicians utilise hand held gamma meters to detect uranium in rock samples, drill cuttings and cores. Borehole geophysical logging equipment typically records the uranium concentration as %eU 3 O8, where e represents an equivalent determination of uranium concentration as opposed to a laboratory assay. This method of uranium determination is an indirect method, as it measures gamma radiation from uranium-238 (U-238) isotope decay chain progeny; principally the bismuth-214 (Bi-214) isotope. Consequently, the uranium determination can be inaccurate due to natural disequilibrium between the U-238 parent and the decay chain progeny. This is especially true in sedimentary hosted uranium deposits, where the uranium and daughter progeny may have been geochemically separated. The gamma detection method for uranium can also be rendered inaccurate by detecting the gamma signature from potassium in clays as well as from thorium; both of which can provide a false (enhanced) eU 3 O8 determination. Prompt Fission Neutron (PFN) technology is a geophysical wireline logging technology used in the same manner as conventional gamma logging. The difference is that PFN provides a direct determination of uranium within a borehole, irrespective of natural disequilibrium or the presence of other radioactive elements. This paper provides a brief description of natural uranium and radioactivity as a basis for explaining the conventional use of gamma radiation detectors for the detection and determination of uranium concentration in exploration boreholes, including the potential pitfalls of this technology. A detailed description of prompt fission neutron technology is also presented, along with a discussion
Kr and Xe isotopes from spontaneous fission of 248Cm and 250Cf
International Nuclear Information System (INIS)
Srinivasan, B.
1980-01-01
Relative yields of Kr and Xe isotopes from the spontaneous fission of 248 Cm and 250 Cf have been determined mass spectrometrically. The yields are as follows: 83 Kr/ 84 Kr/ 85 Kr/ 86 Kr = 0.223/0.458/0.596/ identical 1.00 and 0.306/0.582/0.793/ identical 1.00; 131 Xe/ 134 Xe/ 136 Xe = 0.486/0.819/1.075 identical 1.00 and 0.343/0.506/0.851/ identical 1.00 from 248 Cm and 250 Cf, respectively. The Xe yields from 248 Cm agree with an earlier determination by Leich et al. Neither of these yield patterns matches that of fissiogenic Kr and Xe in carbonaceous chondrites and hence 248 Cm and 250 Cf are ruled out as progenitors of the meteoritic Kr and Xe. In general, none of the spontaneously fissioning nuclides of actinide elements can be identified as a possible progenitor. Even the mixtures of actinides, including a combination of 248 Cm and 250 Cm, are unsuitable. The origin of anomalous Kr and Xe in carbonaceous chondrites must then be traced either to the spontaneous fission of a superheavy element or to peculiarities in specific nucleosynthetic reactions. (orig.)
International Nuclear Information System (INIS)
Anon.
1981-01-01
The method covers the detection and measurement of delayed neutron-emitting fission products contained in nuclear reactor coolant water while the reactor is operating. The method is limited to the measurement of the delayed neutron-emitting bromine isotope of mass 87 and the delayed neutron-emitting iodine isotope of mass 137. The other delayed neutron-emitting fission products cannot be accurately distinguished from nitrogen 17, which is formed under some reactor conditions by neutron irradiation of the coolant water molecules. The method includes a description of significance, measurement variables, interferences, apparatus, sampling, calibration, standardization, sample measurement procedures, system efficiency determination, calculations, and precision
Neutron emission in fission of highly excited californium nuclei (E*=76 MeV)
International Nuclear Information System (INIS)
Blinov, M.V.; Bordyug, V.M.; Kozulin, Eh.M.; Mozhaev, A.N.; Levitovich, M.; Muzychka, Yu.A.; Penionzhkevich, Yu.Eh.; Pustyl'nik, B.I.
1990-01-01
The differential cross sections for neutron production in the fission of highly excited californium nuclei formed in the 238 U+ 12 C (105 MeV) reaction have been measured. From the analysis of the experimental data is follows that the number of pre-fission neutrons substantially exceeds the value obtained in the framework of the standard statistical model. The saddle-to-scission time of the excited nucleus is estimated on the basis of the neutron multiplicity. The dependences of the neutron number and neutron average energies upon the fragment mass are determined
The total kinetic energy release in the fast neutron-induced fission of {sup 232}Th
Energy Technology Data Exchange (ETDEWEB)
King, Jonathan; Yanez, Ricardo; Loveland, Walter; Barrett, J. Spencer; Oscar, Breland [Oregon State University, Dept. of Chemistry, Corvallis, OR (United States); Fotiades, Nikolaos; Tovesson, Fredrik; Young Lee, Hye [Los Alamos National Laboratory, Physics Division, Los Alamos, NM (United States)
2017-12-15
The post-emission total kinetic energy release (TKE) in the neutron-induced fission of {sup 232}Th was measured (using white spectrum neutrons from LANSCE) for neutron energies from E{sub n} = 3 to 91 MeV. In this energy range the average post-neutron total kinetic energy release decreases from 162.3 ± 0.3 at E{sub n} = 3 MeV to 154.9 ± 0.3 MeV at E{sub n} = 91 MeV. Analysis of the fission mass distributions indicates that the decrease in TKE with increasing neutron energy is a combination of increasing yields of symmetric fission (which has a lower associated TKE) and a decrease in the TKE release in asymmetric fission. (orig.)
Measurements of fast neutron-induced fission data of Np-237
Energy Technology Data Exchange (ETDEWEB)
Win, Than; Saito, Keiichiro; Baba, Mamoru; Iwasaki, Tomohiko; Ibaraki, Masanobu; Miura, Takako; Sanami, Toshiya; Nauchi, Yasushi; Hirakawa, Naohiro [Tohoku Univ., Sendai (Japan). Faculty of Engineering
1998-03-01
We have performed the following measurements for {sup 237}Np using the 4.5 MV Dynamitron accelerator of Tohoku University as the pulsed neutron source: (1) Prompt fission neutron spectrum for 0.62 MeV incident neutrons, and (2) Neutron-Induced fission cross-section between 10 and 100 keV. The prompt fission neutron spectrum was measured using TOF method with a heavily shielded NE213 scintillation detector. The Maxwellian temperature T{sub m} derived is 1.28 MeV, which is lower than that of 1.38 MeV in JENDL-3.2. The fission cross sections were measured between 10 - 100 keV. The results are between JENDL-3.2 and ENDF/B-VI. (author)
Consultants' meeting on prompt fission neutron spectra of major actinides. Summary report
International Nuclear Information System (INIS)
Capote Noy, R.; Maslov, V.; Bauge, E.; Ohsawa, T.; Vorobyev, A.; Chadwick, M.B.; Oberstedt, S.
2009-01-01
A Consultants' Meeting on 'Prompt Fission Neutron Spectra of Major Actinides' was held at IAEA Headquarters, Vienna, Austria, to discuss the adequacy and quality of the recommended prompt fission neutron spectra to be found in existing nuclear data applications libraries. These prompt fission neutron spectra were judged to be inadequate, and this problem has proved difficult to resolve by means of theoretical modelling. Major adjustments may be required to ensure the validity of such important data. There is a strong requirement for an international effort to explore and resolve these difficulties and recommend prompt fission neutron spectra and uncertainty covariance matrices for the actinides over the neutron energy range from thermal to 20 MeV. Participants also stressed that there would be a strong need for validation of the resulting data against integral critical assembly and dosimetry data. (author)
Dynamic effects in neutron induced fission of 230Th and 232Th
International Nuclear Information System (INIS)
Trochon, J.; Frehaut, J.; Pranal, Y.; Simon, G.; Boldeman, J.W.
1982-09-01
The fission fragment characteristics of the two thorium isotopes 230 Th and 232 Th have been measured in an attempt to study the evolution of the fissioning nucleus from saddle point to scission. The partial fission channel at the saddle point have been deduced from a fission fragment angular distribution and fission cross section analysis. Changes with energy in the average number of prompt neutron (νsub(p)) emitted per fission and the total fragment kinetic energy (TKE) have been observed in the fission threshold region. A rather good fit of νsub(p) and TKE values has been obtained on the basis of a correlation of these quantities and the partial fission channel ratios. This leads to expect for these isotopes a passage from saddle point to scission sufficiently rapid for the coupling between collective and intrinsic excitation to be very weak [fr
Fission signal detection using helium-4 gas fast neutron scintillation detectors
Energy Technology Data Exchange (ETDEWEB)
Lewis, J. M., E-mail: lewisj@ufl.edu; Kelley, R. P.; Jordan, K. A. [Nuclear Engineering Program, University of Florida, Gainesville, Florida 32611 (United States); Murer, D. [Arktis Radiation Detectors Ltd., 8045 Zurich (Switzerland)
2014-07-07
We demonstrate the unambiguous detection of the fission neutron signal produced in natural uranium during active neutron interrogation using a deuterium-deuterium fusion neutron generator and a high pressure {sup 4}He gas fast neutron scintillation detector. The energy deposition by individual neutrons is quantified, and energy discrimination is used to differentiate the induced fission neutrons from the mono-energetic interrogation neutrons. The detector can discriminate between different incident neutron energies using pulse height discrimination of the slow scintillation component of the elastic scattering interaction between a neutron and the {sup 4}He atom. Energy histograms resulting from this data show the buildup of a detected fission neutron signal at higher energies. The detector is shown here to detect a unique fission neutron signal from a natural uranium sample during active interrogation with a (d, d) neutron generator. This signal path has a direct application to the detection of shielded nuclear material in cargo and air containers. It allows for continuous interrogation and detection while greatly minimizing the potential for false alarms.
Properties of neutron-rich nuclei studied by fission product nuclear chemistry
International Nuclear Information System (INIS)
Meyer, R.A.; Henry, E.A.; Griffin, H.C.; Lien, O.G. III; Lane, S.M.; Stevenson, P.C.; Yaffe, R.P.; Skarnemark, G.
1979-09-01
A review is given of the properties of neutron-rich nuclei studied by fission product nuclear chemistry and includes the techniques used in elemental isolation and current research on the structure of nuclei near 132 Sn, particle emission, and coexisting structure in both neutron-poor and neutron-rich nuclei. 35 references
Energy Technology Data Exchange (ETDEWEB)
Duke, Dana Lynn [Los Alamos National Lab. (LANL), Los Alamos, NM (United States)
2015-11-12
This Ph.D. dissertation describes a measurement of the change in mass distributions and average total kinetic energy (TKE) release with increasing incident neutron energy for fission of ^{235}U and ^{238}U. Although fission was discovered over seventy-five years ago, open questions remain about the physics of the fission process. The energy of the incident neutron, En, changes the division of energy release in the resulting fission fragments, however, the details of energy partitioning remain ambiguous because the nucleus is a many-body quantum system. Creating a full theoretical model is difficult and experimental data to validate existing models are lacking. Additional fission measurements will lead to higher-quality models of the fission process, therefore improving applications such as the development of next-generation nuclear reactors and defense. This work also paves the way for precision experiments such as the Time Projection Chamber (TPC) for fission cross section measurements and the Spectrometer for Ion Determination in Fission (SPIDER) for precision mass yields.
Mass distributions in monoenergetic-neutron-induced fission of 232Th
International Nuclear Information System (INIS)
Glendenin, L.E.; Gindler, J.E.; Ahmad, I.; Henderson, D.J.; Meadows, J.W.
1980-01-01
Fission product yields for 38 masses were determined for the fission of 232 Th with essentially monoenergetic neutrons of 2.0, 3.0, 4.0, 5.9, 6.4, 6.9, 7.6, and 8.0 MeV. Fission product activities were measured by Ge(Li) γ-ray spectrometry of irradiated 232 Th foils and by chemical separation of the fission product elements followed by β counting. The mass yield data for 232 Th(n,f ) show a sensitive increase of fission yields in the near-symmetric mass region (valley) with increasing incident neutron energy E/sub n/ and a pronounced dip in yield at the onset of second-chance fission just above the neutron binding energy (at approx. 6 MeV) where the excitation energy is lowered by competition with neutron evaporation prior to fission. The effect of second-chance fission is also seen in the yields of asymmetric peak products. A distinct third peak is observed at symmetry in the valley of the mass distribution, and enhanced yields are observed in the asymmetric peaks at masses associated with even Z (proton pairing effect). The fission yeilds of 232 Th(n,f ) are compared with those of 238 U(n,f ) and 232 Th
Chatillon, A; Granier, Th; Laurent, B; Taïeb, J; Noda, S; Haight, R C; Devlin, M; Nelson, R O; O’Donnell, J M
2010-01-01
Prompt fission neutron spectra in the neutron-induced fission of 239Pu have been measured for incident neutron energies from 1 to 200 MeV at the Los Alamos Neutron Science Center. Preliminary results are discussed and compared to theoretical model calculation.
Energy Technology Data Exchange (ETDEWEB)
Hirose, K., E-mail: hirose.kentaro@jaea.go.jp [Advanced Science Research Center, Japan Atomic Energy Agency (JAEA), Tokai, Ibaraki 319-1195 (Japan); Nishio, K.; Makii, H.; Nishinaka, I.; Ota, S. [Advanced Science Research Center, Japan Atomic Energy Agency (JAEA), Tokai, Ibaraki 319-1195 (Japan); Nagayama, T. [Advanced Science Research Center, Japan Atomic Energy Agency (JAEA), Tokai, Ibaraki 319-1195 (Japan); Graduate School of Science and Engineering, Ibaraki University, Mito 310-0056 (Japan); Tamura, N. [Advanced Science Research Center, Japan Atomic Energy Agency (JAEA), Tokai, Ibaraki 319-1195 (Japan); Graduate School of Science and Technology, Niigata University, Niigata 950-2181 (Japan); Goto, S. [Graduate School of Science and Technology, Niigata University, Niigata 950-2181 (Japan); Andreyev, A.N. [Advanced Science Research Center, Japan Atomic Energy Agency (JAEA), Tokai, Ibaraki 319-1195 (Japan); Department of Physics, University of York, Heslington, York YO10 5DD (United Kingdom); Vermeulen, M.J. [Advanced Science Research Center, Japan Atomic Energy Agency (JAEA), Tokai, Ibaraki 319-1195 (Japan); Gillespie, S.; Barton, C. [Department of Physics, University of York, Heslington, York YO10 5DD (United Kingdom); Kimura, A.; Harada, H. [Nuclear Science and Engineering Center, JAEA, Tokai, Ibaraki 319-1195 (Japan); Meigo, S. [J-PARC Center, JAEA, Tokai, Ibaraki 319-1195 (Japan); Chiba, S. [Research Laboratory for Nuclear Reactors, Tokyo Institute of Technology, Tokyo 152-8550 (Japan); Ohtsuki, T. [Research Reactor Institute, Kyoto University, Kumatori-cho S' ennangun,Osaka 590-0494 (Japan)
2017-06-01
Fission and capture reactions were simultaneously measured in the neutron-induced reactions of {sup 241}Am at the spallation neutron facility of the Japan Proton Accelerator Research Complex (J-PARC). Data for the neutron energy range of E{sub n}=0.1–20 eV were taken with the TOF method. The fission events were observed by detecting prompt neutrons accompanied by fission using liquid organic scintillators. The capture reaction was measured by detecting γ rays emitted in the deexcitation of the compound nuclei using the same detectors, where the prompt fission neutrons and capture γ rays were separated by a pulse shape analysis. The cross sections were obtained by normalizing the relative yields at the first resonance to evaluations or other experimental data. The ratio of the fission to capture cross sections at each resonance is compared with those from an evaluated nuclear data library and other experimental data. Some differences were found between the present values and the library/literature values at several resonances.
International Nuclear Information System (INIS)
Zheng Wei; Zeen Yao; Changlin Lan; Yan Yan; Yunjian Shi; Siqi Yan; Jie Wang; Junrun Wang; Jingen Chen; Chinese Academy of Sciences, Shanghai
2015-01-01
Monte Carlo transport code Geant4 has been successfully utilised to study of neutron-induced fission reaction for 232 Th in the transport neutrons generated from 3 H(d,n) 4 He neutron source. The purpose of this work is to examine the applicability of Monte Carlo simulations for the computation of fission reaction process. For this, Monte Carlo simulates and calculates the characteristics of fission reaction process of 232 Th(n,f), such as the fission yields distribution, kinetic energy distribution, fission neutron spectrum and decay γ-ray spectrum. This is the first time to simulate the process of neutron-induced fission reaction using Geant4 code. Typical computational results of neutron-induced fission reaction of 232 Th(n,f) reaction are presented. The computational results are compared with the previous experimental data and evaluated nuclear data to confirm the certain physical process model in Geant4 of scientific rationality. (author)
Utilization of fast reactor excess neutrons for burning long-lived fission products
International Nuclear Information System (INIS)
Kawashima, K.; Kobayashi, K.; Kaneto, K.
1995-01-01
An evaluation is made on a large MOX fuel fast reactor's capability of burning long lived fission product Tc-99, which dominates the long term radiotoxicity of the high level radioactive waste. The excess neutrons generated in the fast reactor core are utilized to transmute Tc-99 to stable isotopes due to neutron capture reaction. The fission product target assemblies which consist of Tc-99 are charged to the reactor core periphery. The fission product target neutrons are moderated to a great deal to pursue the possibility of enhancing the transmutation rate. Any impacts of loading the fission product target assemblies on the core nuclear performances are assessed. A long term Tc-99 accumulation scenario is considered in the mix of fission product burner fast reactor and non-burner LWRs. (author)
Detection of fission signatures induced by a low-energy neutron source
International Nuclear Information System (INIS)
Ocherashvili, A.; Becka, A.; Mayorovb, V.; Roesgen, E.; Crochemoreb, J.-M.; Mosconi, M.; Pedersen, B.; Heger, C.
2015-01-01
We present a method for the detection of special nuclear materials (SNM) in shielded containers which is both sensitive and applicable under field conditions. The method uses an external pulsed neutron source to induce fission in SNM and subsequent detection of the fast prompt fission neutrons. The detectors surrounding the container under investigation are liquid scintillation detectors able to distinguish gamma rays from fast neutrons by means of the pulse shape discrimination method (PSD). One advantage of these detectors, besides the ability for PSD analysis, is that the analogue signal from a detection event is of very short duration (typically few tens of nanoseconds). This allows the use of very short coincidence gates for the detection of the prompt fission neutrons in multiple detectors while benefiting from a low accidental (background) coincidence rate yielding a low detection limit. Another principle advantage of this method derives from the fact that the external neutron source is pulsed. By proper time gating the interrogation can be conducted by epithermal and thermal source neutrons only. These source neutrons do not appear in the fast neutron signal following the PSD analysis thus providing a fundamental method for separating the interrogating source neutrons from the sample response in form of fast fission neutrons. The paper describes laboratory tests with a configuration of eight detectors in the Pulsed Neutron Interrogation Test Assembly (PUNITA). The sensitivity of the coincidence signal to fissile mass is investigated for different sample configurations and interrogation regimes.
International Nuclear Information System (INIS)
Wagemans, C.
1991-01-01
Since its discovery in 1946, light (charged) particle accompanied fission (ternary fission) has been extensively studied, for spontaneous as well as for induced fission reactions. The reason for this interest was twofold: the ternary particles being emitted in space and time close to the scission point were expected to supply information on the scission point configuration and the ternary fission process was an important source of helium, tritium, and hydrogen production in nuclear reactors, for which data were requested by the nuclear industry. Significant experimental progress has been realized with the advent of high-resolution detectors, powerful multiparameter data acquisition systems, and intense neutron and photon beams. As far as theory is concerned, the trajectory calculations (in which scission point parameters are deduced from the experimental observations) have been very much improved. An attempt was made to explain ternary particle emission in terms of a Plateau-Rayleigh hydrodynamical instability of a relatively long cylindrical neck or cylindrical nucleus. New results have also been obtained on the so-called open-quotes trueclose quotes ternary fission (fission in three about-equal fragments). The spontaneous emission of charged particles has also clearly been demonstrated in recent years. This chapter discusses the main characteristics of ternary fission, theoretical models, light particle emission probabilities, the dependence of the emission probabilities on experimental variables, light particle energy distributions, light particle angular distributions, correlations between light particle accompanied fission observables, open-quotes trueclose quotes ternary fission, and spontaneous emission of heavy ions. 143 refs., 18 figs., 8 tabs
Neutron analysis of a hybrid system fusion-fission
International Nuclear Information System (INIS)
Dorantes C, J. J.; Francois L, J. L.
2011-11-01
The use of energy at world level implies the decrease of natural resources, reduction of fossil fuels, in particular, and a high environmental impact. In view of this problem, an alternative is the energy production for nuclear means, because up to now is one of the less polluting energy; however, the nuclear fuel wastes continue being even a problem without being solved. For the above mentioned this work intends the creation of a device that incorporates the combined technologies of fission and nuclear fusion, called Nuclear Hybrid Reactor Fusion-Fission (HRFF). The HRFF has been designed theoretically with base in experimental fusion reactors in different parts of the world like: United States, Russia, Japan, China and United Kingdom, mainly. The hybrid reactor model here studied corresponds at the Compact Nuclear Facility Source (CNFS). The importance of the CNFS resides in its feasibility, simple design, minor size and low cost; uses deuterium-tritium like main source of neutrons, and as fuel can use the spent fuel of conventional nuclear reactors, such as the current light water reactors. Due to the high costs of experimental research, this work consists on simulating in computer a proposed model of CNFS under normal conditions of operation, to modify the arrangement of the used fuel: MOX and IMF, to analyze the obtained results and to give final conclusions. In conclusion, the HRFF can be a versatile system for the management of spent fuel of light water reactors, so much for the possibility of actinides destruction, like for the breeding of fissile material. (Author)
Goodness of isospin in neutron rich systems from the fission fragment distribution
Garg, Swati; Jain, Ashok Kumar
2017-09-01
We present the results of our calculations for the relative yields of neutron-rich fission fragments emitted in 208Pb (18O, fission) reaction by using the concept of the conservation of isospin and compare with the experimental data. We take into account a range of isospin values allowed by the isospin algebra and assume that the fission fragments are formed in isobaric analog states. We also take into account the neutron multiplicity data for various neutron-emission channels in each partition, and use them to obtain the weight factors in calculating the yields. We then calculate the relative yields of the fission fragments. Our calculated results are able to reproduce the experimental trends reasonably well. This is the first direct evidence of the isospin conservation in neutron-rich systems and may prove a very useful tool in their studies.
Curves and tables of neutron cross sections of fission product nuclei in JENDL-3
Energy Technology Data Exchange (ETDEWEB)
Nakagawa, Tsuneo [ed.
1992-06-15
Neutron cross sections of 172 nuclei in the fission product region stored in JENDL-3 are shown in graphs and tables. The evaluation work of these nuclei was made by the Fission Product Nuclear Data Working Group of the Japanese Nuclear Data Committee, in the neutron energy region from 10{sup {minus}5} eV to 20 MeV. Almost of the cross section data reproduced in graphs in this report. The cross section averaged over 38 energy intervals are listed in a table. Shown in order tables are thermal cross sections, resonance integrals, Maxwellian neutron flux average cross sections, fission spectrum average cross sections, 14-MeV cross sections, one group average cross sections in neutron flux of typical types of fission reactors and average cross sections in the 30-keV Maxwellian spectrum.
Pulse-shape discrimination in radioanalytical methods. Part I. Delayed fission neutron counting
International Nuclear Information System (INIS)
Posta, S.; Vacik, J.; Hnatowicz, V.; Cervena, J.
1999-01-01
In this study the principle of pulse shape discrimination (PSD) has been employed in delayed fission neutron counting (DNC) method. Effective elimination of unwanted gamma background signals in measured radiation spectra has been proved. (author)
International Nuclear Information System (INIS)
Wagner, M.; Vonach, H.
1990-01-01
These proceedings of a specialists' meeting on neutron activation cross sections for fission and fusion energy applications are divided into 4 sessions bearing on: - data needs: 4 conferences - experimental work: 11 conferences - theoretical work: 4 conferences - evaluation work: 5 conferences
Curves and tables of neutron cross sections of fission product nuclei in JENDL-3
International Nuclear Information System (INIS)
Nakagawa, Tsuneo
1992-06-01
Neutron cross sections of 172 nuclei in the fission product region stored in JENDL-3 are shown in graphs and tables. The evaluation work of these nuclei was made by the Fission Product Nuclear Data Working Group of the Japanese Nuclear Data Committee, in the neutron energy region from 10 -5 eV to 20 MeV. Almost all the cross section data are reproduced in graphs in this report. The cross section averaged over 38 energy intervals are listed in a table. Shown in other tables are thermal cross sections, resonance integrals, Maxwellian neutron flux average cross sections, fission spectrum average cross sections, 14-MeV cross sections, one group average cross sections in neutron flux of typical types of fission reactors and average cross sections in the 30-keV Maxwellian spectrum. (author)
International Nuclear Information System (INIS)
Doerschel, B.; Krusche, M.; Schuricht, V.
1980-01-01
The calibration of a personnel neutron dosemeter in different neutron fields is described. The badge-like dosemeter contains 5 detectors: polycarbonate foil (10 μm, Makrofol KG), 232 Th, natural uranium, natural uranium with boron, and natural uranium with cadmium. Detector sensitivity and calibration factors have been calculated and measured in radiation fields of 252 Cf fission neutrons, WWR-S reactor neutrons with and without Cd and Fe shielding, 3-MeV (d,t) generator neutrons, and 238 PuBe neutrons. Measurement range and achievable accuracy are discussed from the point of view of applying the dosemeter in routine and emergency uses
Time Evolving Fission Chain Theory and Fast Neutron and Gamma-Ray Counting Distributions
International Nuclear Information System (INIS)
Kim, K. S.; Nakae, L. F.; Prasad, M. K.; Snyderman, N. J.; Verbeke, J. M.
2015-01-01
Here, we solve a simple theoretical model of time evolving fission chains due to Feynman that generalizes and asymptotically approaches the point model theory. The point model theory has been used to analyze thermal neutron counting data. This extension of the theory underlies fast counting data for both neutrons and gamma rays from metal systems. Fast neutron and gamma-ray counting is now possible using liquid scintillator arrays with nanosecond time resolution. For individual fission chains, the differential equations describing three correlated probability distributions are solved: the time-dependent internal neutron population, accumulation of fissions in time, and accumulation of leaked neutrons in time. Explicit analytic formulas are given for correlated moments of the time evolving chain populations. The equations for random time gate fast neutron and gamma-ray counting distributions, due to randomly initiated chains, are presented. Correlated moment equations are given for both random time gate and triggered time gate counting. There are explicit formulas for all correlated moments are given up to triple order, for all combinations of correlated fast neutrons and gamma rays. The nonlinear differential equations for probabilities for time dependent fission chain populations have a remarkably simple Monte Carlo realization. A Monte Carlo code was developed for this theory and is shown to statistically realize the solutions to the fission chain theory probability distributions. Combined with random initiation of chains and detection of external quanta, the Monte Carlo code generates time tagged data for neutron and gamma-ray counting and from these data the counting distributions.
International Nuclear Information System (INIS)
Dorlet, J.
1991-01-01
A describing algorithm furnishes the probabilities of having exactly N escaping neutrons in the descent of one fission neutron, using the punctual reactor model. Calculations can be performed even for N-values greater than 1000. Numerical results show that discrete neutrons counting is unfit to obtain the N mean value, even for very far subcritical devices. That mean value is still very used in the existing theoretical studies, because its obvious correlation with the device effective multiplication coefficient. For that reason modelling coincidence neutrons counting is not suitable using statistical moments approach, but only using probabilities it selves [fr
International Nuclear Information System (INIS)
Fukahori, Tokio; Iwamoto, Osamu; Chiba, Satoshi
2003-01-01
For an accelerator-driven nuclear waste transmutation system, it is very important to estimate sub-criticality of core system for feasibility and design study of the system. The fission cross section in the intermediate energy range has an important role. A program FISCAL has been developed to calculate neutron-, proton- and photon-induced fission cross sections in the energy region from several tens of MeV to 3 GeV. FISCAL adopts the systematics considering experimental data for Ag- 243 Am. It is found that unified description of neutron-, proton- and photon-induced fission cross sections is available. (author)
International Nuclear Information System (INIS)
Oswald, R.A.; Lanzl, L.H.; Rozenfeld, M.
1981-01-01
Fission track detectors were applied to a unique problem in neutron dosimetry. Measurements of neutron doses were required at locations within a tumor of 1 cm diameter implanted on the back of a mouse and surrounded by a square array of four 252 Cf medical sources. Measurements made in a tissue-equivalent mouse phantom showed that the neutron dose rate to the center of the tumor was 2.18 rads mg -1 h -1 +- 8.4%. The spatial variation of neutron dose to the tumor ranged from 1.88 to 2.55 rads mg -1 h -1 . These measurements agree with calculated values of neutron dose to those locations in the phantom. Fission track detectors have been found to be a reliable tool for neutron dosimetry for geometries in which one wishes to know neutron dose values which may vary considerably over distances of 1 cm or less
International Nuclear Information System (INIS)
Oswald, R.A.; Lanzl, L.H.; Rozenfeld, M.
1981-01-01
Fission track detectors were applied to a unique problem in neutron dosimetry. Measurements of neutron doses were required at locations within a tumor of 1 cm diameter implanted on the back of a mouse and surrounded by a square array of four 252 Cf medical sources. Measurements made in a tissue-equivalent mouse phantom showed that the neutron dose rate to the center of the tumor was 2.18 rads micrograms-1 h-1 +/- 8.4%. The spatial variation of neutron dose to the tumor ranged from 1.88 to 2.55 rads micrograms-1 h-1. These measurements agree with calculated values of neutron dose to those locations in the phantom. Fission track detectors have been found to be a reliable tool for neutron dosimetry for geometries in which one wishes to know neutron dose values which may vary considerably over distances of 1 cm or less
A fission ionization detector for neutron flux measurements at a spallation source
Energy Technology Data Exchange (ETDEWEB)
Wender, S.A. (Los Alamos National Lab., Los Alamos, NM (United States)); Balestrini, S. (Los Alamos National Lab., Los Alamos, NM (United States)); Brown, A. (Los Alamos National Lab., Los Alamos, NM (United States)); Haight, R.C. (Los Alamos National Lab., Los Alamos, NM (United States)); Laymon, C.M. (Los Alamos National Lab., Los Alamos, NM (United States)); Lee, T.M. (Los Alamos National Lab., Los Alamos, NM (United States)); Lisowski, P.W. (Los Alamos National Lab., Los Alamos, NM (United States)); McCorkle, W. (Los Alamos National Lab., Los Alamos, NM (United States)); Nelson, R.O. (Los Alamos National Lab., Los Alamos, NM (United States)); Parker, W. (Los Alamos National Lab., Los Alamos, NM (United States)); Hill, N.W. (Oak Ridge National Lab., Oak Ridge, TN (United States))
1993-11-15
The construction of a neutron flux monitor that can measure absolute neutron intensities in the neutron energy range from below 1 MeV to over 500 MeV is described. The detector consists of an ionization chamber with several thin deposits of fissionable material. The ionization chamber is thin enough that it does not significantly affect the neutron beam and may be left in the neutron flight path during experimental measurements to continuously monitor the beam flux. The use of this monitor at the continuous-energy spallation neutron source at the WNR target area at LAMPF is described. (orig.)
A fission ionization detector for neutron flux measurements at a spallation source
International Nuclear Information System (INIS)
Wender, S.A.; Balestrini, S.; Brown, A.; Haight, R.C.; Laymon, C.M.; Lee, T.M.; Lisowski, P.W.; McCorkle, W.; Nelson, R.O.; Parker, W.; Hill, N.W.
1993-01-01
The construction of a neutron flux monitor that can measure absolute neutron intensities in the neutron energy range from below 1 MeV to over 500 MeV is described. The detector consists of an ionization chamber with several thin deposits of fissionable material. The ionization chamber is thin enough that it does not significantly affect the neutron beam and may be left in the neutron flight path during experimental measurements to continuously monitor the beam flux. The use of this monitor at the continuous-energy spallation neutron source at the WNR target area at LAMPF is described. (orig.)
Development of a “Fission-proxy” Method for the Measurement of 14-MeV Neutron Fission Yields at CAMS
Energy Technology Data Exchange (ETDEWEB)
Gharibyan, Narek [Lawrence Livermore National Lab. (LLNL), Livermore, CA (United States)
2016-10-25
Relative fission yield measurements were made for 50 fission products from 25.6±0.5 MeV alpha-induced fission of Th-232. Quantitative comparison of these experimentally measured fission yields with the evaluated fission yields from 14-MeV neutron-induced fission of U-235 demonstrates the feasibility of the proposed fission-proxy method. This new technique, based on the Bohr-independence hypothesis, permits the measurement of fission yields from an alternate reaction pathway (Th-232 + 25.6 MeV α → U-236* vs. U-235 + 14-MeV n → U-236*) given that the fission process associated with the same compound nucleus is independent of its formation. Other suitable systems that can potentially be investigated in this manner include (but are not limited to) Pu-239 and U-237.
Energy Technology Data Exchange (ETDEWEB)
Gaeggeler, H W [Paul Scherrer Inst. (PSI), Villigen (Switzerland)
1996-11-01
Three different non-diffractive applications of neutrons are outlined, neutron activation analysis, production of radionuclides, mostly for medical applications, and production of short-lived fission nuclides with a so-called gas-jet. It is shown that all three devices may be incorporated into one single insert at SINQ due to their different requests with respect to thermal neutron flux. Some applications of these three facilities are summarized. (author) 3 figs., 1 tab., 8 refs.
International Nuclear Information System (INIS)
Gaeggeler, H.W.
1996-01-01
Three different non-diffractive applications of neutrons are outlined, neutron activation analysis, production of radionuclides, mostly for medical applications, and production of short-lived fission nuclides with a so-called gas-jet. It is shown that all three devices may be incorporated into one single insert at SINQ due to their different requests with respect to thermal neutron flux. Some applications of these three facilities are summarized. (author) 3 figs., 1 tab., 8 refs
Refinements in the Los Alamos model of the prompt fission neutron spectrum
Energy Technology Data Exchange (ETDEWEB)
Madland, D.G., E-mail: dgm@lanl.gov; Kahler, A.C.
2017-01-15
This paper presents a number of refinements to the original Los Alamos model of the prompt fission neutron spectrum and average prompt neutron multiplicity as derived in 1982. The four refinements are due to new measurements of the spectrum and related fission observables many of which were not available in 1982. They are also due to a number of detailed studies and comparisons of the model with previous and present experimental results including not only the differential spectrum, but also integral cross sections measured in the field of the differential spectrum. The four refinements are (a) separate neutron contributions in binary fission, (b) departure from statistical equilibrium at scission, (c) fission-fragment nuclear level-density models, and (d) center-of-mass anisotropy. With these refinements, for the first time, good agreement has been obtained for both differential and integral measurements using the same Los Alamos model spectrum.
Design of In-vessel neutron monitor using micro fission chambers for ITER
International Nuclear Information System (INIS)
Nishitani, Takeo; Kasai, Satoshi
2001-10-01
A neutron monitor using micro fission chambers to be installed inside the vacuum vessel has been designed for compact ITER (ITER-FEAT). We investigated the responses of the micro fission chambers to find the suitable position of micro fission chambers by a neutron Monte Carlo calculation using MCNP version 4b code. It was found that the averaged output of the micro fission chambers behind blankets at upper outboard and lower outboard is insensitive to the changes in the plasma position and the neutron source profile. A set of 235 U micro fission chamber and ''blank'' detector which is a fissile material free detector to identify noise issues such as from γ-rays are installed behind blankets. Employing both pulse counting mode and Campbelling mode in the electronics, the ITER requirement of 10 7 dynamic range with 1 ms temporal resolution can be accomplished. The in-situ calibration has been simulated by MCNP calculation, where a point source of 14 MeV neutrons is moving on the plasma axis. It was found that the direct calibration is possible by using a neutron generator with an intensity of 10 11 n/s. The micro fission chamber system can meet the required 10% accuracy for a fusion power monitor. (author)
Active-interrogation measurements of fast neutrons from induced fission in low-enriched uranium
International Nuclear Information System (INIS)
Dolan, J.L.; Marcath, M.J.; Flaska, M.; Pozzi, S.A.; Chichester, D.L.; Tomanin, A.; Peerani, P.
2014-01-01
A detection system was designed with MCNPX-PoliMi to measure induced-fission neutrons from U-235 and U-238 using active interrogation. Measurements were then performed with this system at the Joint Research Centre in Ispra, Italy on low-enriched uranium samples. Liquid scintillators measured induced fission neutrons to characterize the samples in terms of their uranium mass and enrichment. Results are presented to investigate and support the use of organic liquid scintillators with active interrogation techniques to characterize uranium containing materials. -- Highlights: • We studied low-enriched uranium using active-interrogation experiments including a deuterium–tritium neutron generator and an americium–lithium isotopic neutron source. • Liquid scintillators measured induced-fission neutrons from the active-interrogation methods. • Fast-neutron (DT) and thermal-neutron (Am–Li) interrogation resulted in the measurement of trends in uranium mass and 235 U enrichment respectively. • MCNPX-PoliMi, the Monte Carlo transport code, simulated the measured induced-fission neutron trends in the liquid scintillators
Active-interrogation measurements of fast neutrons from induced fission in low-enriched uranium
Energy Technology Data Exchange (ETDEWEB)
Dolan, J.L., E-mail: jldolan@umich.edu [Department of Nuclear Engineering and Radiological Sciences, University of Michigan, Ann Arbor, MI 48109 (United States); Marcath, M.J.; Flaska, M.; Pozzi, S.A. [Department of Nuclear Engineering and Radiological Sciences, University of Michigan, Ann Arbor, MI 48109 (United States); Chichester, D.L. [Idaho National Laboratory, Idaho Falls, ID 83415 (United States); Tomanin, A.; Peerani, P. [European Commission, Joint Research Centre, Institute for Transuranium Elements, Ispra (Italy)
2014-02-21
A detection system was designed with MCNPX-PoliMi to measure induced-fission neutrons from U-235 and U-238 using active interrogation. Measurements were then performed with this system at the Joint Research Centre in Ispra, Italy on low-enriched uranium samples. Liquid scintillators measured induced fission neutrons to characterize the samples in terms of their uranium mass and enrichment. Results are presented to investigate and support the use of organic liquid scintillators with active interrogation techniques to characterize uranium containing materials. -- Highlights: • We studied low-enriched uranium using active-interrogation experiments including a deuterium–tritium neutron generator and an americium–lithium isotopic neutron source. • Liquid scintillators measured induced-fission neutrons from the active-interrogation methods. • Fast-neutron (DT) and thermal-neutron (Am–Li) interrogation resulted in the measurement of trends in uranium mass and {sup 235}U enrichment respectively. • MCNPX-PoliMi, the Monte Carlo transport code, simulated the measured induced-fission neutron trends in the liquid scintillators.
Transmutation and neutron flux studies with fission chambers in the MEGAPIE target
International Nuclear Information System (INIS)
Chabod, S.; Foucher, Y.; Letourneau, A.; Marie, F.; Toussaint, J.C.; Blandin, Ch.; Chartier, F.; Fioni, G.
2005-01-01
Eight fission micro chambers will be inserted inside the central rod of the 1 MW liquid Pb-Bi MEGAPIE target in order to study the transmutation of two major actinides and to measure the neutron flux at a level of 5%. These chambers were developed for high neutron fluxes and tested at Laue Langevin Institute. (authors)
Measurement of the 235U/238U fission cross section ratio in the 235U fission neutron spectrum
International Nuclear Information System (INIS)
Azimi-Garakani, D.; Bagheri-Darbandi, M.
1983-06-01
Fission cross section ratio of 235 U to 238 U has been measured in the fast neutron field generated by the 235 U fission plate installed on the thermal column of the Tehran Research Reactor (TRR) with a Makrofol solid state nuclear track detector. The experiments were carried out with a set of total six enriched 235 U and depleted 238 U deposits with different masses and Makrofol films of 0.025mm and 0.060mm thicknesses. The chemically etched tracks were counted by an optical microscope. No significant differences were observed with the thin and the thick films. The results showed that the average fission cross section ratio is 3.83+-0.25. (author)
Directory of Open Access Journals (Sweden)
Schmidt K.-H.
2010-10-01
Full Text Available A new model description of fission-fragment yields and prompt neutron emission is developed. The yields of the different fission channels and their properties are attributed to the number of relevant states above the potential-energy landscape on the fission path at the moment of dynamical freeze-out, which is specific to the collective coordinate considered. The model combines well established ideas with novel concepts. The separability principle of macroscopic properties of the compound nucleus and microscopic properties of the fragments strongly reduces the number of model parameters and assures a high predictive power. The recently discovered energy-sorting mechanism in superfluid nuclear dynamics determines the sharing of intrinsic excitation energy at scission and the enhancement of even-odd structure in asymmetric splits.
An evaporation-based model of thermal neutron induced ternary fission of plutonium
International Nuclear Information System (INIS)
Lestone, J.P.
2008-01-01
Ternary fission probabilities for thermal neutron induced fission of plutonium are analyzed within the framework of an evaporation-based model where the complexity of time-varying potentials, associated with the neck collapse, are included in a simplistic fashion. If the nuclear temperature at scission and the fission-neck-collapse time are assumed to be ~ 1.2 MeV and ~ 10 -22 s, respectively, then calculated relative probabilities of ternary-fission light-charged-particle emission follow the trends seen in the experimental data. The ability of this model to reproduce ternary fission probabilities spanning seven orders of magnitude for a wide range of light-particle charges and masses implies that ternary fission is caused by the coupling of an evaporation-like process with the rapid re-arrangement of the nuclear fluid following scission. (author)
Solid State Track Recorder fission rate measurements at high neutron fluence and high temperature
International Nuclear Information System (INIS)
Ruddy, F.H.; Roberts, J.H.; Gold, R.
1985-01-01
Solid State Track Recorder (SSTR) techniques have been used to measure 239-Pu, 235-U, and 237-Np fission rates for total neutron fluences approaching 5 x 10 17 n/cm 2 at temperatures in the range 680 to 830 0 F. Natural quartz crystal SSTRs were used to withstand the high temperature environment and ultra low-mass fissionable deposits of the three isotopes were required to yield scannable track densities at the high neutron fluences. The results of these high temperature, high neutron fluence measurements are reported
Tovesson, F.; Duke, D.; Geppert-Kleinrath, V.; Manning, B.; Mayorov, D.; Mosby, S.; Schmitt, K.
2018-03-01
Different aspects of the nuclear fission process have been studied at Los Alamos Neutron Science Center (LANSCE) using various instruments and experimental techniques. Properties of the fragments emitted in fission have been investigated using Frisch-grid ionization chambers, a Time Projection Chamber (TPC), and the SPIDER instrument which employs the 2v-2E method. These instruments and experimental techniques have been used to determine fission product mass yields, the energy dependent total kinetic energy (TKE) release, and anisotropy in neutron-induced fission of U-235, U-238 and Pu-239.
Edwards, E R; Cassata, W S; Velsko, C A; Yeamans, C B; Shaughnessy, D A
2016-11-01
Precisely-known fission yield distributions are needed to determine a fissioning isotope and the incident neutron energy in nuclear security applications. 14 MeV neutrons from DT fusion at the National Ignition Facility induce fission in depleted uranium contained in the target assembly hohlraum. The fission yields of Kr isotopes (85m, 87, 88, and 89) are measured relative to the cumulative yield of 88 Kr and compared to previously tabulated values. The results from this experiment and England and Rider are in agreement, except for the 85m Kr/ 88 Kr ratio, which may be the result of incorrect nuclear data.
International Nuclear Information System (INIS)
Chatillon, A.; Belier, G.; Granier, T.; Laurent, B.; Morillon, B.; Taieb, J.; Haight, R.C.; Devlin, M.; Nelson, R.O.; Noda, R.S.; O'Donnell, J.M.
2014-01-01
Prompt fission neutron spectra in the neutron-induced fission of "2"3"9Pu have been measured for incident neutron energies from 1 to 200 MeV at the Los Alamos Neutron Science Center. Mean energies deduced from the prompt fission neutron spectra (PFNS) lead to the observation of the opening of the second chance fission at 7 MeV and to indications for the openings of fission channels of third and fourth chances. Moreover, the general trend of the measured PFNS is well reproduced by the different models. The comparison between data and models presents, however, two discrepancies. First, the prompt neutron mean energy seems constant for neutron energy, at least up to 7 MeV, whereas in the theoretical calculations it is continuously increasing. Second, data disagree with models on the shape of the high energy part of the PFNS, where our data suggest a softer spectrum than the predictions. (authors)
International Nuclear Information System (INIS)
Fourmentel, D.; Filliatre, P.; Barbot, L.; Villard, J.-F.; Lyoussi, A.; Geslot, B.; Malo, J.-Y.; Carcreff, H.; Reynard-Carette, C.
2013-06-01
Thermal neutron flux is one of the most important nuclear parameter to be measured on-line in Material Testing Reactors (MTRs). In particular two types of sensors with different physical operating principles are commonly used: self-powered neutron detectors (SPND) and fission chambers with uranium 235 coating. This work aims to compare on one hand the thermal neutron flux evaluation given by these two types of sensors and on the other hand to compare these evaluations with activation dosimeter measurements, which are considered as the reference for absolute neutron flux assessment. This study was conducted in an irradiation experiment, called CARMEN-1, performed during 2012 in OSIRIS reactor (CEA Saclay - France). The CARMEN-1 experiment aims to improve the neutron and photon flux and nuclear heating measurements in MTRs. In this paper we focus on the thermal neutron flux measurements performed in CARMEN-1 experiment. The use of fission chambers to measure the absolute thermal neutron flux in MTRs is not very usual. An innovative calibration method for fission chambers operated in Campbell mode has been developed at the CEA Cadarache (France) and tested for the first time in the CARMEN-1 experiment. The results of these measurements are discussed, with the objective to measure with the best accuracy the thermal neutron flux in the future Jules Horowitz Reactor. (authors)
First wall material damage induced by fusion-fission neutron environment
Energy Technology Data Exchange (ETDEWEB)
Khripunov, Vladimir, E-mail: Khripunov_VI@nrcki.ru
2016-11-01
Highlights: • The highest damage and gas production rates are experienced within the first wall materials of a hybrid fusion-fission system. • About ∼2 times higher dpa and 4–5 higher He appm are expected compared to the values distinctive for a pure fusion system at the same DT-neutron wall loading. • The specific nuclear heating may be increased by a factor of ∼8–9 due to fusion and fission neutrons radiation capture in metal components of the first wall. - Abstract: Neutronic performance and inventory analyses were conducted to quantify the damage and gas production rates in candidate materials when used in a fusion-fission hybrid system first wall (FW). The structural materials considered are austenitic SS, Cu-alloy and V- alloys. Plasma facing materials included Be, and CFC composite and W. It is shown that the highest damage rates and gas particles production in materials are experienced within the FW region of a hybrid similar to a pure fusion system. They are greatly influenced by a combined neutron energy spectrum formed by the two-component fusion-fission neutron source in front of the FW and in a subcritical fission blanket behind. These characteristics are non-linear functions of the fission neutron source intensity. Atomic displacement damage production rate in the FW materials of a subcritical system (at the safe subcriticality limit of ∼0.95 and the neutron multiplication factor of ∼20) is almost ∼2 times higher compared to the values distinctive for a pure fusion system at the same 14 MeV neutron FW loading. Both hydrogen (H) and helium (He) gas production rates are practically on the same level except of about ∼4–5 times higher He-production in austenitic and reduced activation ferritic martensitic steels. A proper simulation of the damage environment in hybrid systems is required to evaluate the expected material performance and the structural component residence times.
Dose-effect relationship of apoptosis induced by fission-neutron in murine thymocytes
International Nuclear Information System (INIS)
Yuan Bin; Li Liang; Xue Wencheng; Sun Jianmin; Wang Baoqin
2000-01-01
Objective: To investigate the effectiveness of high LET fission-neutron to induce apoptosis in murine thymocytes and to compare it with that of low LET 60 Co γ-ray. Methods: Apoptosis induction was studied qualitatively by light and transmission electron microscopy and DNA gel electrophoresis,also quantitatively by flow cytometry(FCM) and diphenylamine (DPA)methods. Results: DNA ladders of murine thymocytes were detectable, the typical apoptosis of thymocytes could be observed morphologically by means of light and electron microscopy at 6 h after fission-neutron irradiation with doses ranging from 0.5 to 5.0 Gy, meanwhile the percentages of apoptosis increased with increasing doses. After exposure to γ-rays with doses ranging from 1.0 to 30 Gy, the experimental results were similar to those from neutron radiation. The incidence of apoptosis peaked at about 20 Gy, the percentages did not increase further when doses increased. Conclusion: Apoptosis of murine thymocytes can be induced when mice are exposed to either fission-neutron (0.5-5.0 Gy) or to γ-ray (1-30 Gy). Although the relationship between apoptosis and radiation doses is similar, the percentage of apoptosis induced by neutron irradiation is higher than that induced by γ-irradiation. The RBE values of fission-neutron for inducing apoptosis murine thymocytes are 2.09 (by FCM method) and 2.37 (by DPA method), respectively. These results also suggest that fission-neutron-induced murine immune tissue is more severe than that induced by γ-rays at several hours post-irradiation and this might be the basis for heavy damage to immune tissues induced by fission-neutron-irradiation in later period
The evaluated neutron cross sections and resonance integrals of fission products with Z = 57-62
International Nuclear Information System (INIS)
Fedorova, A.F.; Pisanko, Zh.I.; Novoselov, G.M.
1976-01-01
Neutron cross sections at a neutron velocity of V=2200 m/s, and resonance integrals for fission products with Z=57-71 are estimated. In obtaining the recommended values the results of the neutron cross sections and resonance integrals for elements used as references were normalized in accordance with the latest adjusted values. In the course of estimation, preference was given to the more accurate methods for obtaining the measured values and to the more recent investigations
New Beta-delayed Neutron Measurements in the Light-mass Fission Group
Energy Technology Data Exchange (ETDEWEB)
Agramunt, J. [Instituto de Física Corpuscular, CSIC-Univ. Valencia, Apdo. Correos 22085, E-46071 Valencia (Spain); García, A.R. [Centro de Investigaciones Energéticas, Medioambientales y Tecnológicas, E-28040 Madrid (Spain); Algora, A. [Instituto de Física Corpuscular, CSIC-Univ. Valencia, Apdo. Correos 22085, E-46071 Valencia (Spain); Äystö, J. [University of Jyväskylä, FI-40014 Jyväskyä (Finland); Caballero-Folch, R.; Calviño, F. [Secció d' Enginyeria Nuclear, Universitat Politécnica de Catalunya, E-08028 Barcelona (Spain); Cano-Ott, D. [Centro de Investigaciones Energéticas, Medioambientales y Tecnológicas, E-28040 Madrid (Spain); Cortés, G. [Secció d' Enginyeria Nuclear, Universitat Politécnica de Catalunya, E-08028 Barcelona (Spain); Domingo-Pardo, C. [Instituto de Física Corpuscular, CSIC-Univ. Valencia, Apdo. Correos 22085, E-46071 Valencia (Spain); Eronen, T. [University of Jyväskylä, FI-40014 Jyväskyä (Finland); Gelletly, W. [Department of Physics, University of Surrey, Guildford GU2 7XH (United Kingdom); Gómez-Hornillos, M.B. [Secció d' Enginyeria Nuclear, Universitat Politécnica de Catalunya, E-08028 Barcelona (Spain); and others
2014-06-15
A new accurate determination of beta-delayed neutron emission probabilities from nuclei in the low mass region of the light fission group has been performed. The measurements were carried out using the BELEN 4π neutron counter at the IGISOL-JYFL mass separator in combination with a Penning trap. The new results significantly improve the uncertainties of neutron emission probabilities for {sup 91}Br, {sup 86}As, {sup 85}As, and {sup 85}Ge nuclei.
The evaluated neutron cross sections and resonance integrals of fission products with Z=63-71
International Nuclear Information System (INIS)
Fedorova, A.F.; Pisanko, Zh.I.; Novoselov, G.M.
1976-01-01
Neutron cross sections at a neutron velocity of V=2200 m/s, and the resonance integrals for fission products with Z=63-71 are estimated. In obtaining the recommended values the results were normalized of the neutron cross sections and resonance integrals for elements used as references in accordance with the latest adjusted values. In the course of estimation, preference was given to the more accurate measuring methods and the more recent investigations. Scientific publications up to 1975 have been used
International Nuclear Information System (INIS)
Naqvi, A.A.
1980-03-01
Fission fragment properties such as mass distribution, kinetic energy distribution or number of prompt emitted neutrons as a function of fragment mass can be used to characterize the scission point configuration. The present experiment allows for the first time to investigate these quantities for neutron induced fission in the MeV range. In this way the influence of excitation energy of the saddle point deformation of the fissioning system ( 237 Np + n) can be studied. Neutrons with energies of 0.8 and 5.5 MeV were produced by the Karlsruhe pulsed 3MV Van de Graaff accelerator. Kinetic energies and velocities of correlated fragments were determined by solid state detectors using the time-of-flight technique. The experimentally determined distributions of fragment properties were compared to a recent model suggested by Wilkins et al. which assumes only relatively weak coupling between internal and collective degrees of freedom. At least qualitative agreement is found for most of the results. (orig.) [de
The LANL/LLNL Program to Measure Prompt Fission Neutron Spectra at LANSCE
Haight, Robert; Wu, Ching Yen; Lee, Hye Young; Taddeucci, Terry; Mosby, Shea; O'Donnell, John; Fotiades, Nikolaos; Devlin, Mattew; Ullmann, John; Nelson, Ronald; Wender, Stephen; White, Morgan; Solomon, Clell; Neudecker, Denise; Talou, Patrick; Rising, Michael; Bucher, Brian; Buckner, Matthew; Henderson, Roger
2015-10-01
Accurate data on the spectrum of neutrons emitted in neutron-induced fission are needed for applications and for a better understanding of the fission process. At LANSCE we have made important progress in understanding systematic uncertainties and in obtaining data for 235U on the low-energy part of the prompt fission neutron spectra (PFNS), a particularly difficult region because down-scattered neutrons go in this direction. We use a double time-of-flight technique to determine energies of incoming and outgoing neutrons. With data acquisition via waveform digitizers, accidental coincidences between fission chamber and neutron detector are measured to high statistical accuracy and then subtracted from measured events. Monte Carlo simulations with high performance computers have proven to be essential in the design to minimize neutron scattering and in calculating detector response. Results from one of three approaches to analyzing the data will be presented. This work is funded by the US Department of Energy, National Nuclear Security Administration and Office of Nuclear Physics.
Symmetry of neutron-induced 235U fission at individual resonances. III
Energy Technology Data Exchange (ETDEWEB)
Cowan, G A; Bayhurst, B P; Prestwood, R J; Gilmore, J S; Knobeloch, G W [Los Alamos Scientific Laboratory, University of California, Los Alamos, NM (United States)
1970-05-15
A number of experiments have been described in recent years which document variations in the yields of symmetric or near-symmetric fission products at resonances in 235-U and 239-Pu neutron-induced fission. In the case of 239-Pu fission it has been demonstrated in a statistically significant sample of s-wave neutron resonances (J{sup {pi}} = 0{sup +} or 1{sup +}) that the 0{sup +} levels have a characteristic 115Cd yield which is a factor of four higher than the yield at 1{sup +} levels. The fission widths of the J = 0 levels are larger than the J = 1 levels by a factor of ten. The populations of the two groups are in reasonable agreement with the expected (2J + 1) distributions. Previous efforts to obtain equally detailed data in 235-U fission and 233-U fission by the 'wheel' technique have not been entirely successful due in large part to the high level densities in the epithermal excitation functions of these nuclides and the consequent difficulty in characterizing fission yields in a sufficiently large and well-resolved sample of levels. In a recent 'wheel' experiment (late summer, 1969) vith a 235-U target the energy resolution was sufficiently improved in the region 20 eV-60 eV to allow characterization of a sample of 38 reasonably well-resolved levels by their relative symmetry of fission. (author)
International Nuclear Information System (INIS)
Heinisch, H.L.; Hamilton, M.L.; Sommer, W.F.; Ferguson, P.D.
1992-01-01
The objective of this work is to investigate the effects of the neutron energy spectrum in low dose irradiations on the microstructures and mechanical properties of metals. Radiation effects due to low doses of spallation neutrons are compared directly to those produced by fission and fusion neutrons. Yield stress changes of pure Cu, alumina-dispersion-strengthened Cu and AISI 316 stainless steel irradiated at 36-55 C in the Los Alamos Spallation Radiation Effects Facility (LASREF) are compared with earlier results of irradiations at 90 C using 14 MeV D-T fusion neutrons at the Rotating Target Neutron Source and fission reactor neutrons in the Omega West Reactor. At doses up to 0.04 displacements per atom (dpa), the yield stress changes due to the three quite different neutron spectra correlate well on the basis of dpa in the stainless steel and the Cu alloy. However, in pure Cu, the measured yield stress changes due to spallation neutrons were anomalously small and should be verified by additional irradiations. With the exception of pure Cu, the low dose, low temperature experiments reveal no fundamental differences in radiation hardening by fission, fusion or spallation neutrons when compared on the basis of dpa
International Nuclear Information System (INIS)
Volkov, V.V.; Cherepanov, E.A.; Kalandarov, Sh.A.
2016-01-01
A new approach to the interpretation of the process of spontaneous fission of heavy nuclei is suggested. It is based on nuclear physics data which are obtained in heavy ion collisions. The process of spontaneous fission consists of three sequential stages: clusterization of the valent nucleons of a heavy nucleus into a light nucleus-cluster, which leads to the formation of a dinuclear system; evolution of the dinuclear system which proceeds by nucleon transfer from the heavy to light nucleus; and decay of the dinuclear system from the equilibrium configuration into two fragments. [ru
A delayed neutron technique for measuring induced fission rates in fresh and burnt LWR fuel
Energy Technology Data Exchange (ETDEWEB)
Jordan, K.A., E-mail: kajordan@gmail.co [Paul Scherrer Institut, Laboratory for Reactor Physics and System Behaviour, 5232 Villigen (Switzerland); Perret, G. [Paul Scherrer Institut, Laboratory for Reactor Physics and System Behaviour, 5232 Villigen (Switzerland)
2011-04-01
The LIFE-PROTEUS program at the Paul Scherrer Institut is being undertaken to characterize the interfaces between burnt and fresh fuel assemblies in modern LWRs. Techniques are being developed to measure fission rates in burnt fuel following re-irradiation in the zero-power PROTEUS research reactor. One such technique utilizes the measurement of delayed neutrons. To demonstrate the feasibility of the delayed neutron technique, fresh and burnt UO{sub 2} fuel samples were irradiated in different positions in the PROTEUS reactor, and their neutron outputs were recorded shortly after irradiation. Fission rate ratios of the same sample irradiated in two different positions (inter-positional) and of two different samples irradiated in the same position (inter-sample) were derived from the measurements and compared with Monte Carlo predictions. Derivation of fission rate ratios from the delayed neutron measured signal requires correcting the signal for the delayed neutron source properties, the efficiency of the measurement setup, and the time dependency of the signal. In particular, delayed neutron source properties strongly depend on the fissile and fertile isotopes present in the irradiated sample and must be accounted for when deriving inter-sample fission rate ratios. Measured inter-positional fission rate ratios generally agree within 1{sigma} uncertainty (on the order of 1.0%) with the calculation predictions. For a particular irradiation position, however, a bias of about 2% is observed and is currently under investigation. Calculated and measured inter-sample fission rate ratios have C/E values deviating from unity by less than 1% and within 2{sigma} of the statistical uncertainties. Uncertainty arising from delayed neutron data is also assessed, and is found to give an additional 3% uncertainty factor. The measurement data indicate that uncertainty is overestimated.
Measurement of mass distribution of U-235 fission products in the intermediate neutron region
International Nuclear Information System (INIS)
Nakagomi, Yoshihiro; Kobayashi, Shohei; Yamamoto, Shuji; Kanno, Ikuo; Wakabayashi, Hiroaki.
1982-01-01
The mass distribution and the momentum distribution of U-235 fission products in the intermediate neutron region were measured by using a combination system of the Yayoi intermediate neutron column and an electron linear accelerator. The double energy measurement method was applied. A fission chamber, which consists of an enriched uranium target and two Si surface barrier detectors, was used for the measurement of the neutrons with energy above 1.3 eV. The linear accelerator was operated at the repetition rate of 100 Hz and the pulse width of 10 ns. The data obtained by the two-dimensional pulse height analysis were analyzed by the Schmitt's method. The preliminary results of the mass distribution and the momentum distribution of fission fragments were obtained. (Kato, T.)
Energy Technology Data Exchange (ETDEWEB)
Abramo; vich, S.N.; Andreev, M.F.; Bol`shakov, Y.M. [Institute of Experimental Physics, Arzamas (Russian Federation)] [and others
1995-10-01
Measurements have been carried out of {sup 238}Np fission cross-section by thermal neutrons. The isotope {sup 238}Np was built up through the reaction {sup 238}U(p,n) on an electrostatic accelerator. Extraction and cleaning of the sample were done by ion-exchange chromatography. Fast neutrons were generated on the electrostatic accelerator through the reaction {sup 9}Be(d,n); a polyethylene block was used to slow down neutrons. Registration of fission fragments was performed with dielectric track detectors. Suggesting that the behavior of {sup 238}Np and {sup 238}U. Westscott`s factors are indentical the fission cross-section of {sup 238}Np was obtained: {sigma}{sub fo}=2110 {plus_minus} 75 barn.
Energy Technology Data Exchange (ETDEWEB)
Lau, Ch
2000-09-15
This work is a contribution to the PARRNe project (production of radioactive neutron-rich isotopes). This project is based on the fission fragments coming from the fission of 238-uranium induced by fast neutrons. The fast neutron flux is produced by the collisions of deutons in a converter. Thick targets of uranium carbide and liquid uranium targets have been designed in order to allow a quick release of fission fragments. A device, able to trap on a cryogenic thimble rare gas released by the target, has allowed the production of radioactive nuclei whose half-life is about 1 second. This installation has been settled to different deuton accelerators in the framework of the European collaboration SPIRAL-2. A calibration experiment has proved the feasibility of fixing an ISOL-type isotope separator to a 15 MV tandem accelerator, this installation can provide 500 nA deutons beams whose energy is 26 MeV and be a valuable tool for studying fast-neutron induced fission. Zinc, krypton, rubidium, cadmium, iodine, xenon and cesium beams have been produced in this installation. The most intense beams reach 10000 nuclei by micro-coulomb for 26 MeV deutons. An extra gain of 2 magnitude orders can be obtained by using a more specific ion source and by increasing the thickness of the target. Another extra gain of 2 magnitude orders involves 100 MeV deutons.
Independent yields of Rb and Cs isotopes from thermal-neutron induced fission of 235U
International Nuclear Information System (INIS)
Balestrini, S.J.; Decker, R.; Wollnik, H.; Wuensch, K.D.; Jung, G.; Koglin, E.; Siegert, G.
1979-01-01
The relative yields of Rb and Cs isotopes from thermal-neutron fission of 235 U have been redetermined using the mass separator OSTIS, on-line at a neutron guide of the High-Flux Beam Reactor at the Institut Laue-Langevin, Grenoble, France. The separator ion source was a hot oven containing 235 U in a graphite matrix. The neutron beam was pulsed. Alkali fission products diffused out of the graphite and were ionized, thus producing a stepwise increase in the analyzed ion beam proportional to the independent fission yield. The ion beam and the fissions in the source were monitored simultaneously. The diffusion of Rb and Cs from the source was exponential in time with half-lives ranging from 2.8 to 18 sec, depending upon the element and source temperature. The independent fission yields of Rb and Cs are normalized by equating their element yields to each other and to a value computed from the charge distributions observed with the recoil separator LOHENGRIN and well established mass yields. Fractional independent yields are deduced from the independent fission yields, and these compare very well with the EOZ model described by Wahl
Measurement of fast neutron induced fission cross section of minor-actinide
International Nuclear Information System (INIS)
Hirakawa, Naohiro
2000-06-01
In fuel cycles with recycled actinide, core characteristics are largely influenced by minor actinide (MA: Np, Am, Cm). Accurate nuclear data of MA such as fission cross section are required to estimate the effect of MA with high accuracy. In this study, fast neutron induced fission cross section of MA is measured using Dynamitron accelerator in Tohoku University. The followings were performed in this fiscal year; (1) Research of nuclear data of MA, (2) Sample preparation and sample mass assay, (3) Investigation of neutron sources with the energy of several 10 keV, (4) Preliminary measurement of fission cross section using Dynamitron accelerator. As the result, four 237 Np samples were prepared and the sample mass were measured using alpha-spectrometry with the accuracy of 1.2%. Then, it was confirmed that a neutron source via 7 Li(p,n) 7 Be reaction using a Li-thick target is suitable for measuring fission cross section of MA in the energy region of several 10 keV. Furthermore, it was verified by the preliminary measurement that the measurement of fission cross section of MA is available using a fission chamber and electronics developed in this study. (author)
Energy Technology Data Exchange (ETDEWEB)
Trahan, Alexis Chanel [Los Alamos National Lab. (LANL), Los Alamos, NM (United States)
2017-09-15
The objectives of this presentation are to introduce the basic physics of neutron production, interactions and detection; identify the processes that generate neutrons; explain the most common neutron mechanism, spontaneous and induced fission and (a,n) reactions; describe the properties of neutron from different sources; recognize advantages of neutron measurements techniques; recognize common neutrons interactions; explain neutron cross section measurements; describe the fundamental of ^{3}He detector function and designs; and differentiate between passive and active assay techniques.
Evidence of pair correlations in actinide neutron-induced fission cross sections
International Nuclear Information System (INIS)
Maslov, V.M.
2000-01-01
It is shown that irregularities in fission cross sections in MeV incident neutron energy region could be attributed to the interplay of few-quasiparticle excitations in the level density of the fissioning and residual nuclei. It is suggested the intrinsic quasiparticle state density modelling approach both at stable and saddle-point deformations. The experimental manifestation of few-quasiparticle irregularities in the level density depends on the fission barrier structure and internal excitation energy at the saddle point, corresponding to the higher barrier hump. The explicit evidence is observed in case of fissile and non-fissile target nuclides [ru
International Nuclear Information System (INIS)
Dickens, J.K.; Emery, J.F.; Love, T.A.; McConnell, J.W.; Northcutt, K.J.; Peelle, R.W.; Weaver, H.
1977-10-01
Fission-product decay energy-releases rates were measured for thermal-neutron fission of 235 U. Samples of mass 1 to 10 μg were irradiated for 1 to 100 sec by use of the fast pneumatic-tube facility at the Oak Ridge Research Reactor. The resulting beta- and gamma-ray emissions were counted for times-after-fission between 2 and 14,000 seconds. The data were obtained for beta and gamma rays separately as spectral distributions, N(E/sub γ/) vs E/sub γ/ and N(E/sub beta/) vs E/sub β/. For the gamma-ray data the spectra were obtained by using a NaI detector, while for the beta-ray data the spectra were obtained by using an NE-110 detector with an anticoincidence mantle. The raw data were unfolded to provide spectral distributions of modest resolution. These were integrated over E/sub γ/ and E/sub β/ to provide total yield and energy integrals as a function of time after fission. Results are low compared to the present 1973 ANS Decay-heat standard. A complete description of the experimental apparatus and data-reduction techniques is presented. The final integral data are given in tabular and graphical form and are compared with published data. 41 figures, 13 tables
Study of asymmetric fission yield behavior from neutron-deficient Hg isotope
International Nuclear Information System (INIS)
Perkasa, Y. S.; Waris, A.; Kurniadi, R.; Su'ud, Z.
2014-01-01
A study of asymmetric fission yield behavior from a neutron-deficient Hg isotope has been conducted. The fission yield calculation of the neutron-deficient Hg isotope using Brownian Metropolis shape had showed unusual result at decreasing energy. In this paper, this interesting feature will be validated by using nine degree of scission shapes parameterization from Brosa model that had been implemented in TALYS nuclear reaction code. This validation is intended to show agreement between both model and the experiment result. The expected result from these models considered to be different due to dynamical properties that implemented in both models
Energy Technology Data Exchange (ETDEWEB)
Mushtaq, A. [Isotope Production Division, Pakistan Institute of Nuclear Science and Technology, P.O. Nilore, Islamabad (Pakistan)], E-mail: mushtaqa@pinstech.org.pk; Iqbal, Massod; Bokhari, Ishtiaq Hussain; Mahmood, Tariq; Mahmood, Tayyab; Ahmad, Zahoor; Zaman, Qamar [Nuclear Engineering Division, Pakistan Institute of Nuclear Science and Technology, P.O. Nilore, Islamabad (Pakistan)
2008-02-15
Neutronic and thermal hydraulic analysis for the fission molybdenum-99 production at PARR-1 has been performed. Low enriched uranium foil (<20% {sup 235}U) will be used as target material. Annular target designed by ANL (USA) will be irradiated in PARR-1 for the production of 100 Ci of molybdenum-99 at the end of irradiation, which will be sufficient to prepare required {sup 99}Mo/{sup 99m}Tc generators at PINSTECH and its supply in the country. Neutronic and thermal hydraulic analysis were performed using various codes. Data shows that annular targets can be safely irradiated in PARR-1 for production of required amount of fission molybdenum-99.
Study of the production of neutron-rich isotope beams issuing from fissions induced by fast neutrons
International Nuclear Information System (INIS)
Lau, Ch.
2000-01-01
This work is a contribution to the PARRNe project (production of radioactive neutron-rich isotopes). This project is based on the fission fragments coming from the fission of 238-uranium induced by fast neutrons. The fast neutron flux is produced by the collisions of deutons in a converter. Thick targets of uranium carbide and liquid uranium targets have been designed in order to allow a quick release of fission fragments. A device, able to trap on a cryogenic thimble rare gas released by the target, has allowed the production of radioactive nuclei whose half-life is about 1 second. This installation has been settled to different deuton accelerators in the framework of the European collaboration SPIRAL-2. A calibration experiment has proved the feasibility of fixing an ISOL-type isotope separator to a 15 MV tandem accelerator, this installation can provide 500 nA deutons beams whose energy is 26 MeV and be a valuable tool for studying fast-neutron induced fission. Zinc, krypton, rubidium, cadmium, iodine, xenon and cesium beams have been produced in this installation. The most intense beams reach 10000 nuclei by micro-coulomb for 26 MeV deutons. An extra gain of 2 magnitude orders can be obtained by using a more specific ion source and by increasing the thickness of the target. Another extra gain of 2 magnitude orders involves 100 MeV deutons
International Nuclear Information System (INIS)
Osorio, A.M.; Hadler, J.C.; Iunes, P.J.; Paulo, S.R. de
1993-06-01
In order to use the fission track dating method the flux gradient was verified within the sample holder, in some irradiation positions of the IEA-R1 reactor at IPEN/CNEN, Sao Paulo. The fission track dating method considers only the thermal neutron fission tracks, to subtract the other contributions sample irradiations with a cadmium cover was performed. The neutron flux cadmium influence was studied. (author)
International Nuclear Information System (INIS)
Stewart, L.
1979-03-01
In response to an action by the Standards Subcommittee of the Cross Section Evaluation Working Group, a workshop was convened to determine the status of available information on prompt fission neutron spectra. The experimental data were reviewed and theoretical models were developed. The current ENDF/B fission neutron spectra files were summarized. Further work is currently under way, especially to provide a better theoretical tool to represent energy-dependent fission spectra. 5 references
Neutron induced fission of 237Np – status, challenges and opportunities
Directory of Open Access Journals (Sweden)
Ruskov Ivan
2018-01-01
Full Text Available Nowadays, there is an increased interest in a complete study of the neutron-induced fission of 237Np. This is due to the need of accurate and reliable nuclear data for nuclear science and technology. 237Np is generated (and accumulated in the nuclear reactor core during reactor operation. As one of the most abundant long-lived isotopes in spent fuel (“waste”, the incineration of 237Np becomes an important issue. One scenario for burning of 237Np and other radio-toxic minor actinides suggests they are to be mixed into the fuel of future fast-neutron reactors, employing the so-called transmutation and partitioning technology. For testing present fission models, which are at the basis of new generation nuclear reactor developments, highly accurate and detailed neutron-induced nuclear reaction data is needed. However, the EXFOR nuclear database for 237Np on neutron-induced capture cross-section, σγ, and fission cross-section, σf, as well as on the characteristics of capture and fission resonance parameters (Γγ, Γf, σoΓf, fragments mass-energy yield distributions, multiplicities of neutrons vn and γ-rays vγ, has not been updated for decades.
Radioactive ion beams produced by neutron-induced fission at ISOLDE
Catherall, R; Gilardoni, S S; Köster, U
2003-01-01
The production rates of neutron-rich fission products for the next-generation radioactive beam facility EURISOL are mainly limited by the maximum amount of power deposited by protons in the target. An alternative approach is to use neutron beams to induce fission in actinide targets. This has the advantage of reducing: the energy deposited by the proton beam in the target; contamination from neutron-deficient isobars that would be produced by spallation; and mechanical stress on the target. At ISOLDE CERN, tests have been made on standard ISOLDE actinide targets using fast neutron bunches produced by bombarding thick, high-Z metal converters with 1 and 1.4 GeV proton pulses. This paper reviews the first applications of converters used at ISOLDE. It highlights the different geometries and the techniques used to compare fission yields produced by the proton beam directly on the target with neutron-induced fission. Results from the six targets already tested, namely UC2/graphite and ThO2 targets with tungsten an...
Wilson, J N; Halipre, P; Oberstedt, S; Oberstedt, A
2014-01-01
At the IPN Orsay we have developed a unique, directional, fast neutron source called LICORNE, intended initially to facilitate prompt fission gamma measurements. The ability of the IPN Orsay tandem accelerator to produce intense beams of $^7$Li is exploited to produce quasi-monoenergetic neutrons between 0.5 - 4 MeV using the p($^7$Li,$^7$Be)n inverse reaction. The available fluxes of up to 7 × 10$^7$ neutrons/second/steradian for the thickest hydrogen-rich targets are comparable to similar installations, but with two added advantages: (i) The kinematic focusing produces a natural neutron beam collimation which allows placement of gamma detectors adjacent to the irradiated sample unimpeded by source neutrons. (ii) The background of scattered neutrons in the experimental hall is drastically reduced. The dedicated neutron converter was commissioned in June 2013. Some preliminary results from the first experiment using the LICORNE neutron source at the IPN Orsay are presented. Prompt fission gamma rays from fas...
International Nuclear Information System (INIS)
Noda, S.; Haight, R. C.; Nelson, R. O.; Devlin, M.; O'Donnell, J. M.; Chatillon, A.; Granier, T.; Belier, G.; Taieb, J.; Kawano, T.; Talou, P.
2011-01-01
Prompt fission neutron spectra from 235 U and 239 Pu were measured for incident neutron energies from 1 to 200 MeV at the Weapons Neutron Research facility (WNR) of the Los Alamos Neutron Science Center, and the experimental data were analyzed with the Los Alamos model for the incident neutron energies of 1-8 MeV. A CEA multiple-foil fission chamber containing deposits of 100 mg 235 U and 90 mg 239 Pu detected fission events. Outgoing neutrons were detected by the Fast Neutron-Induced γ-Ray Observer array of 20 liquid organic scintillators. A double time-of-flight technique was used to deduce the neutron incident energies from the spallation target and the outgoing energies from the fission chamber. These data were used for testing the Los Alamos model, and the total kinetic energy parameters were optimized to obtain a best fit to the data. The prompt fission neutron spectra were also compared with the Evaluated Nuclear Data File (ENDF/B-VII.0). We calculate average energies from both experimental and calculated fission neutron spectra.
The 235U Prompt Fission Neutron Spectrum in the BR1 Reactor at SCK•CEN
Wagemans, Jan; Malambu, Edouard; Borms, Luc; Fiorito, Luca
2016-02-01
The BR1 research reactor at SCK•CEN has a spherical cavity in the graphite above the reactor core. In this cavity an accurately characterised Maxwellian thermal neutron field is present. Different converters can be loaded in the cavity in order to obtain other types of neutron (and gamma) irradiation fields. Inside the so-called MARK III converter a fast 235U(n,f) prompt fission neutron field can be obtained. With the support of MCNP calculations, irradiations in MARK III can be directly related to the pure 235U(n,f) prompt fission neutron spectrum. For this purpose MARK III spectrum averaged cross sections for the most relevant fluence dosimetry reactions have been determined. A calibration factor for absolute measurements has been determined applying activation dosimetry following ISO/IEC 17025 standards.
The 235U Prompt Fission Neutron Spectrum in the BR1 Reactor at SCK•CEN
Directory of Open Access Journals (Sweden)
Wagemans Jan
2016-01-01
Full Text Available The BR1 research reactor at SCK•CEN has a spherical cavity in the graphite above the reactor core. In this cavity an accurately characterised Maxwellian thermal neutron field is present. Different converters can be loaded in the cavity in order to obtain other types of neutron (and gamma irradiation fields. Inside the so-called MARK III converter a fast 235U(n,f prompt fission neutron field can be obtained. With the support of MCNP calculations, irradiations in MARK III can be directly related to the pure 235U(n,f prompt fission neutron spectrum. For this purpose MARK III spectrum averaged cross sections for the most relevant fluence dosimetry reactions have been determined. A calibration factor for absolute measurements has been determined applying activation dosimetry following ISO/IEC 17025 standards.
International Nuclear Information System (INIS)
Gundorin, N.A.; Kopach, Y.N.; Telezhnikov, S.A.
1994-01-01
The independent yields of 239 Pu fission fragments by means of gamma-spectroscopy method were measured for light and heavy groups on the IBR-30 reactor in Dubna. Comparative analysis of experimental data for fission induced by thermal and resonance neutrons was performed. The possibilities to increase the measurement's precision consist of the employment of a HPGe detector with high efficiency and its open-quotes activeclose quotes shielding in the gamma spectrometer, as well as a high speed electronics system. In this way the number of identified fragments will be increased and independent yields will be measured to a precision of 1-3%. Measurements at the source with shorter neutron pulse duration to increase neutron energy resolution will be possible after the reconstruction of a modern neutron source in Dubna in accordance with the IREN project
Effect of high gamma background on neutron sensitivity of fission detectors
International Nuclear Information System (INIS)
Balagi, V.; Prasad, K.R.; Kataria, S.K.
2004-01-01
Tests were performed on two parallel plate and two cylindrical fission detectors in pulse and dc mode. The effect of gamma background on neutron sensitivity was studied in thermal neutron flux from 30 nv to 60 nv over which gamma field intensity ranging from 230 kR/h to 3.7 MR/h was superposed. In the case of one of the parallel plate detectors the fall in neutron sensitivity was observed to be 3.7% at 1 MR/h and negligible below 1 MR/h. In the case of one of the cylindrical counters the fall in neutron sensitivity was negligible below 500 kR/h and 37% at 1 MR/h. The data was used to derive the design parameters for a wide range fission detector to be procured for PFBR instrumentation for operation at 600 degC and gamma background of 1 MR/h. (author)
Study of the neutron-photon competition during fission fragment de-excitation
International Nuclear Information System (INIS)
Min, Dong Pil.
1976-01-01
A program was developed to study in detail the competition between neutron and photon emissions during the different stages of the nucleus de-excitation. The main conclusions of this work are the following: the neutron-photon competition fairly depends of the initial spin of the primary fragment. It has a strong effect on the mean number of emitted neutrons, on the photon energy, and to a lower degree, on the mean energy per neutron. A relation between the mean initial spin of the heavy fragment for the almost symmetrical fission, the mean initial spin of the heavy fragment for a very asymmetric fission and the corresponding values of the mean number of emitted neutrons is given. The mean initial excitation energy must increase of about 9MeV for the nucleus to emit one more neutron. Two reasons are given to explain the fact that the measured neutron multiplicity variance is higher for the heavy fragment than for the light one: either the existence of a covariance between spin and excitation energy distribution, or a dispersion of the values of the mean number of emitted neutrons due to the mass and charge distribution resulting from experimental incertitudes. The mean energy per neutron calculated with the program is in good agreement with measured values [fr
Directory of Open Access Journals (Sweden)
de France G.
2014-03-01
Full Text Available A combination of germanium detectors has been installed at the PF1B neutron guide of the ILL to perform the prompt spectroscopy of neutron-rich nuclei produced in the neutron-capture induced-fission of 235U and 241Pu. In addition LaBr3 detectors from the FATIMA collaboration have been installed in complement with the EXOGAM clovers to measure lifetimes of low-lying excited states. The measured characteristics and online spectra indicate very good performances of the overall setup.
Teratogenic and embryolethal effects in mice of fission-spectrum neutrons and γ-rays
International Nuclear Information System (INIS)
Cairnie, A.B.; Grahn, D.; Rayburn, H.B.; Williamson, F.S.; Brown, R.J.
1974-01-01
Fission-spectrum neutrons from the Janus reactor at Argonne National Laboratory were compared with γ-rays in terms of their relative biological effectiveness (RBE) for embryolethal and teratogenic effects in mice. No evidence was found of any processes that were abnormally sensitive to neutrons. The RBE for killing embryos and producing abnormal embryos or specific abnormalities was between 2 and 3. This is close to the values found in other systems for processes involving cell killing. (U.S.)
Neutron Diffusion in a Space Lattice of Fissionable and Absorbing Materials
Feynman, R. P.; Welton, T. A.
1946-08-27
Methods are developed for estimating the effect on a critical assembly of fabricating it as a lattice rather than in the more simply interpreted homogeneous manner. An idealized case is discussed supposing an infinite medium in which fission, elastic scattering and absorption can occur, neutrons of only one velocity present, and the neutron m.f.p. independent of position and equal to unity with the unit of length used.
Neutron rich clusters and the dynamics of fission and fusion
International Nuclear Information System (INIS)
Armbruster, P.
1988-07-01
In this lecture I want to discuss experimental evidence for the appearance of cluster aspects in the dynamics of large rearrangement processes, as fusion and fission. Clusters in the sense as used in my lecture are the strongly bound doubly magic nuclei as 20 Ca 28 48 , 28 Ni 50 78 , 132 50 Sn 82 , and 208 82 Pb 126 and the superheavy nucleus 298 114 184 . Two of these nuclei, 78 Ni and 298 114 have not yet been identified. I discuss first the experimental findings from heavy element production. Then I cover the stability of cluster aspects to intrinsic excitation energy in fusion and fission. (orig./HSI)
International Nuclear Information System (INIS)
Lang, G.P.
1980-12-01
This study is concerned with the engineering aspects of the transmutation of fission products utilizing neutrons generated in fusion reactors. It is assumed that fusion reactors, although not yet developed, will be available around the turn of the century. Therefore, early studies of this type are appropriate as a guide to the large amount of further investigations that will be needed to fully evaluate this concept. Not all of the radioactive products from light water reactors can be economically transmuted, but it appears that the most hazardous can. This requires that fission-product wastes must first be separated into a number of fractions, and in some instances this must be accomplished with extremely high separation factors. A review of current commercial separation processes and of promising methods that are now in the laboratory stage indicate that the necessary processes can most likely be developed but will require an active and sustained development program. Current fusion reactor concepts were examined as to their suitability for transmuting the separated fission wastes. It was concluded that the long-lived fission products were most amenable to transmutation. The medium-lived fission products, Cs-137 and Sr-90, require higher neutron fluxes than are available in the most developed fusion reactor concepts. Concepts which are less developed may eventually be adaptable as transmuters of these fission products
Beta-delayed fission and neutron emission calculations for the actinide cosmochronometers
International Nuclear Information System (INIS)
Meyer, B.S.; Howard, W.M.; Mathews, G.J.; Takahashi, K.; Moeller, P.; Leander, G.A.
1989-01-01
The Gamow-Teller beta-strength distributions for 19 neutron-rich nuclei, including ten of interest for the production of the actinide cosmochronometers, are computed microscopically with a code that treats nuclear deformation explicitly. The strength distributions are then used to calculate the beta-delayed fission, neutron emission, and gamma deexcitation probabilities for these nuclei. Fission is treated both in the complete damping and WKB approximations for penetrabilities through the nuclear potential-energy surface. The resulting fission probabilities differ by factors of 2 to 3 or more from the results of previous calculations using microscopically computed beta-strength distributions around the region of greatest interest for production of the cosmochronometers. The indications are that a consistent treatment of nuclear deformation, fission barriers, and beta-strength functions is important in the calculation of delayed fission probabilities and the production of the actinide cosmochronometers. Since we show that the results are very sensitive to relatively small changes in model assumptions, large chronometric ages for the Galaxy based upon high beta-delayed fission probabilities derived from an inconsistent set of nuclear data calculations must be considered quite uncertain
Measurement of fast neutron induced fission cross section of minor-actinide
International Nuclear Information System (INIS)
Hirakawa, Naohiro
1997-03-01
In fuel cycles with recycled actinide, core characteristics are largely influenced by minor actinide (MA: Np, Am, Cm). Accurate nuclear data of MA such as fission cross section are required to estimate the effect of MA with high accuracy. In this study, fast neutron induced fission cross section of MA is measured using Dynamitron Accelerator in Tohoku University. The experimental method and the samples, which were developed or introduced during the last year, were improved in this fiscal year: (1) Development of a sealed fission chamber, (2) Intensification of Li neutron target, (3) Improvement of time-resolution of Time-of-Flight (TOF) electronic circuit, (4) Introduction of Np237 samples with large sample mass and (5) Introduction of a U235 sample with high purity. Using these improved tools and samples, the fission cross section ratio of Np237 relative to U235 was measured between 5 to 100 keV, and the fission cross section of Np237 was deduced. On the other hand, samples of Am241 and Am243 were obtained from Japan Atomic Energy Research Institute (JAERI) after investigating fission cross section of two americium isotopes (Am241 and Am 243) which are important for core physics calculation of fast reactors. (author)
Energy Technology Data Exchange (ETDEWEB)
Mueller, J.M., E-mail: jonathan_mueller@ncsu.edu; Mattingly, J.
2016-07-21
There is a significant and well-known anisotropy between the prompt neutrons emitted from a single fission event; these neutrons are most likely to be observed at angles near 0° or 180° relative to each other. However, the propagation of this anisotropy through different generations of a fission chain reaction has not been previously studied. We have measured this anisotropy in neutron–neutron coincidences from a subcritical highly-multiplying assembly of plutonium metal. The assembly was a 4.5 kg α-phase plutonium metal sphere composed of 94% {sup 239}Pu and 6% {sup 240}Pu by mass. Data were collected using two EJ-309 liquid scintillators and two EJ-299 plastic scintillators. The angular distribution of neutron–neutron coincidences was measured at 90° and 180° and found to be largely isotropic. Simulations were performed using MCNPX-PoliMi of similar plutonium metal spheres of varying sizes and a correlation between the neutron multiplication of the assembly and the anisotropy of neutron–neutron coincidences was observed. In principle, this correlation could be used to assess the neutron multiplication of an unknown assembly.
Fifth International Conference on Fission and Properties of Neutron-Rich Nuclei
Ramayya, A V; ICFN5
2014-01-01
These proceedings are the fifth in the series of International Conferences covering fission and properties of neutron-rich nuclei, which are at the forefront of nuclear research. The time interval of 5 years between each conference allows for significant new results to be achieved. Recently, world leaders in theory and experiments in research and the development of new facilities for research presented their latest results in areas such as synthesis of superheavy elements, new facilities for and recent results with radioactive ion beams, structure of neutron-rich nuclei, nuclear fission process, fission yields and nuclear astrophysics. This book is a major source of the latest research in these areas and plans for the future. The conference brought together a unique group of over 100 speakers including leaders from the major nuclear laboratories in Canada, China, France, Finland, Germany, Italy, Japan, Russia, Switerzland and the US along with leading research scientists from around the world.
Analysis of 137Cs in fission based neutron dosimetry
International Nuclear Information System (INIS)
Peltonen, T.
1995-11-01
137 Cs analysis is based on dissolving an irradiated fission dosimeter and chemically separating the cesium from the rest of the fission material. The samples consisted of uranium and neptunium in the form of metal or oxide. The uranium samples were dissolved in nitric acid and the neptunium samples in a mixture of nitric acid and chloric acid with addition of hydrogen peroxide. Cs was precipitated into a mixture of ammonium molyndophoshate and cellulose powder. A preparate for measurement was made from the precipitate and covered with polyethen plastic. Since other fission products than cesium were precipitated as well from the more recently irradiated samples, the activity measurements could not be carried out with a NaI(Tl) cavity crystal, but had to be made with a less efficient but more selective germanium semiconductor crystal. The method is well suited for 137 Cs determination, especially for older dosimeters where the more short-lived fission products have decayed. (orig.) (6 refs., 7 figs., 7 tabs.)
Energy balance in MeV neutron induced fission
International Nuclear Information System (INIS)
Ruben, A.; Maerten, H.; Deeliger, D.
1992-01-01
In this paper, general trends of energy balance changes with increasing incidence energy are described in the framework of a simple scission point model including semi-empirical temperature-dependent shell correction energies. In particular, the different behavior of the total kinetic energy (TKE) dependence for several fissioning nuclei (Th, U, Pu) is explained
Preliminary results of total kinetic energy modelling for neutron-induced fission
International Nuclear Information System (INIS)
Visan, I.; Giubega, G.; Tudora, A.
2015-01-01
The total kinetic energy as a function of fission fragments mass TKE(A) is an important quantity entering in prompt emission calculations. The experimentally distributions of TKE(A) are referring to a limited number of fission systems and incident energies. In the present paper, a preliminary model for TKE calculation in neutron induced fission system is presented. The range of fission fragments is chosen as in the Point by Point treatment. The model needs as input only mass excesses and deformation parameters taken from available nuclear databases being based on the following approximations: total excitation energy of fully accelerated fission fragments TXE is calculated from energy balance of neutron-induced fission systems as sum of the total excitation energy at scission E*sciss and deformation energy Edef. The deformation energy at scission is given by minimizing the potential energy at the scission configuration. At the scission point, the fission system is described by two spheroidal fragments nearly touching by a pre-scission distance or neck caused by the nuclear forces between fragments. Therefore, the Columbian repulsion depending on neck and, consequently, on the fragments deformation at scission, is essentially in TKE determination. An approximation is made based on the fission modes. For the very symmetric fission, the dominant super long channel is characterized by long distance between fragments leading to low TKE values. Due to magic and double-magic shells closure, the dominant S1 fission mode for pairs with heavy fragment mass AH around 130-134 is characterized by spherical heavy fragment shape and easily deformed light fragment. The nearly spherical shape of the complementary fragments are characterized by minimum distance, and consequently to maximum TKE values. The results obtained for TKE(A) are in good agreement with existing experimental data for many neutron induced fission systems, e.g. ''2''3''3&apos
14.2 MeV neutron induced U-235 fission cross section measurement
International Nuclear Information System (INIS)
Li Jingwen; Shen Guanren; Ye Zongyuan; Li Anli; Zhou Shuhua; Sun Zhongfan; Wu Jingxia; Huang Tanzi
1986-01-01
The cross section of U-235 fission induced by 14.2 MeV neutrons was measured by the time correlated associated particle method. The result obtained is (2.078+-0.040) barn. Comparison with other author's is also given. (author)
Group Representation of the Prompt Fission Neutron Spectrum of {sup 252}Cf
Energy Technology Data Exchange (ETDEWEB)
Croft, S.; Miller, K. A. [Safeguards Science and Technology Group (N-1), Nuclear Nonproliferation Division, Los Alamos National Laboratory, Los Alamos(United States)
2011-12-15
We review the spectral representation used for the prompt fission neutron spectrum of 252Cf in the International Organization for Standardization document ISO 8529-1. We find corrections to Table A.2, the discrete group structure form, of this report are needed. We describe the approach to generating replacement values and provide a new tabulation.
Studying fission neutrons with 2E-2v and 2E
Directory of Open Access Journals (Sweden)
Al-Adili Ali
2018-01-01
The 2E technique utilizes an ionization chamber together with two liquid scintillator detectors. Two measurements have been performed, one of 252Cf(sf and another one of thermal-neutron induced fission in 235U(n,f. Results from 252Cf(sf are reported here.
The Prompt Fission Neutron Spectrum of 235U for Einc 0.7-5.0 MeV
Energy Technology Data Exchange (ETDEWEB)
Gomez, Jaime A. [Los Alamos National Lab. (LANL), Los Alamos, NM (United States); Devlin, Matthew James [Los Alamos National Lab. (LANL), Los Alamos, NM (United States); Haight, Robert Cameron [Los Alamos National Lab. (LANL), Los Alamos, NM (United States); O' Donnell, John M. [Los Alamos National Lab. (LANL), Los Alamos, NM (United States); Lee, Hye Young [Los Alamos National Lab. (LANL), Los Alamos, NM (United States); Mosby, Shea Morgan [Los Alamos National Lab. (LANL), Los Alamos, NM (United States); Taddeucci, Terry Nicholas [Los Alamos National Lab. (LANL), Los Alamos, NM (United States); Kelly, Keegan John [Los Alamos National Lab. (LANL), Los Alamos, NM (United States); Fotiadis, Nikolaos [Los Alamos National Lab. (LANL), Los Alamos, NM (United States); Neudecker, Denise [Los Alamos National Lab. (LANL), Los Alamos, NM (United States); White, Morgan Curtis [Los Alamos National Lab. (LANL), Los Alamos, NM (United States); Talou, Patrick [Los Alamos National Lab. (LANL), Los Alamos, NM (United States); Rising, Michael Evan [Los Alamos National Lab. (LANL), Los Alamos, NM (United States); Solomon, Clell Jeffrey Jr. [Los Alamos National Lab. (LANL), Los Alamos, NM (United States); Wu, Ching-Yen [Lawrence Livermore National Lab. (LLNL), Livermore, CA (United States); Bucher, Brian Michael [Lawrence Livermore National Lab. (LLNL), Livermore, CA (United States); Buckner, Matthew Quinn [Lawrence Livermore National Lab. (LLNL), Livermore, CA (United States); Henderson, Roger Alan [Lawrence Livermore National Lab. (LLNL), Livermore, CA (United States)
2017-03-23
The Chi-Nu experiment aims to accurately measure the prompt fission neutron spectrum (PFNS) for the major actinides. At the Los Alamos Neutron Science Center (LANSCE), fission can be induced using the white neutron source. Using a two arm time of flight (T.O.F) technique; Chi-Nu presents a preliminary result of the low energy component of the 235U PFNS measured using an array of 22-Lithium glass scintillators.
Status report on the development of a prompt fission neutron uranium borehole logging technique
International Nuclear Information System (INIS)
Smith, G.W.
1977-05-01
The prompt fission neutron (PFN) method of direct uranium measurement was studied. The PFN uranium logging technique measures the enhanced epithermal neutron population created by the prompt thermal fission of 235 U to assay uranium mineralization around a borehole. This neutron population exists for several hundred microseconds after a pulsed neutron source produces a burst of high energy (14 MeV) neutrons. A feasibility study established the basic relationship between the uranium concentration and the enhanced epithermal neutron count, and defined the major measurement perturbing factors. Following the feasibility study, development of a PFN prototype field probe was undertaken. A laboratory type neutron generator, the Controlatron, was modified for use in the probe. Field evaluation of the prototype system began in January 1976. Comparisons of neutron logs and natural gamma logs taken during this evaluation period clearly define many disequilibrium conditions as verified by ore grade estimates from core samples. The feasibility of the PFN logging technique to detect uranium in-situ has now been demonstrated
Preliminary neutronics calculation of fusion-fission hybrid reactor breeding spent fuel assembly
International Nuclear Information System (INIS)
Ma Xubo; Chen Yixue; Gao Bin
2013-01-01
The possibility of using the fusion-fission hybrid reactor breeding spent fuel in PWR was preliminarily studied in this paper. According to the fusion-fission hybrid reactor breeding spent fuel characteristics, PWR assembly including fusion-fission hybrid reactor breeding spent fuel was designed. The parameters such as fuel temperature coefficient, moderator temperature coefficient and their variation were investigated. Results show that the neutron properties of uranium-based assembly and hybrid reactor breeding spent fuel assembly are similar. The design of this paper has a smaller uniformity coefficient of power at the same fissile isotope mass percentage. The results will provide technical support for the future fusion-fission hybrid reactor and PWR combined with cycle system. (authors)
Electron spin resonance of gamma, electron, neutron and fission fragments irradiated K2SO4
International Nuclear Information System (INIS)
Kamali, J.; Walton, G.N.
1985-01-01
The electron spin resonance (ESR) of K 2 SO 4 irradiated by γ, electron, neutron and fission fragments has been investigated. The ESR spectra are attributed mainly to the formation of SO 3 - , SO 4 - , SO 2 - , and O 3 - radical ions. The most intense radical ion observed was due to the SO 3 - , and the other radicals were relatively much lower in intensity. Thermal annealing showed a significant decrease in the concentration of radical ions. The concentration of SO 3 - was measured in γ-irradiated K 2 SO 4 and K 2 SO 4 containing fission fragments. In fission fragments irradiated K 2 SO 4 , the G-value observed for SO 3 - radical formation was about eight times higher than that of γ-irradiated K 2 SO 4 . This was attributed to the high LET (Linear Energy Transfer) of the fission fragments. (author)
Fission Product Yields from {sup 232}Th, {sup 238}U, and {sup 235}U Using 14 MeV Neutrons
Energy Technology Data Exchange (ETDEWEB)
Pierson, B.D., E-mail: bpnuke@umich.edu [Department of Nuclear Engineering Radiological Sciences, University of Michigan, 2355 Bonisteel Blvd., Ann Arbor, MI 48109 (United States); Pacific Northwest National Laboratory, P.O. Box 999, Richland, WA 99352 (United States); Greenwood, L.R. [Pacific Northwest National Laboratory, P.O. Box 999, Richland, WA 99352 (United States); Flaska, M. [Department of Mechanical and Nuclear Engineering, Pennsylvania State University, 227 Reber Bldg., University Park, PA 16802 (United States); Pozzi, S.A. [Department of Nuclear Engineering Radiological Sciences, University of Michigan, 2355 Bonisteel Blvd., Ann Arbor, MI 48109 (United States)
2017-01-15
Neutron-induced fission yield studies using deuterium-tritium fusion-produced 14 MeV neutrons have not yet directly measured fission yields from fission products with half-lives on the order of seconds (far from the line of nuclear stability). Fundamental data of this nature are important for improving and validating the current models of the nuclear fission process. Cyclic neutron activation analysis (CNAA) was performed on three actinide targets–thorium-oxide, depleted uranium metal, and highly enriched uranium metal–at the University of Michigan's Neutron Science Laboratory (UM-NSL) using a pneumatic system and Thermo-Scientific D711 accelerator-based fusion neutron generator. This was done to measure the fission yields of short-lived fission products and to examine the differences between the delayed fission product signatures of the three actinides. The measured data were compared against previously published results for {sup 89}Kr, −90, and −92 and {sup 138}Xe, −139, and −140. The average percent deviation of the measured values from the Evaluated Nuclear Data Files VII.1 (ENDF/B-VII.1) for thorium, depleted-uranium, and highly-enriched uranium were −10.2%, 4.5%, and −12.9%, respectively. In addition to the measurements of the six known fission products, 23 new fission yield measurements from {sup 84}As to {sup 146}La are presented.
Determination of 233U, 235U, 238U and 239Pu fission yields induced by fission and 14.7 MeV neutrons
International Nuclear Information System (INIS)
Laurec, Jean; Adam, Albert; Bruyne, Thierry de.
1981-12-01
The 233 U, 235 U, 238 U, 239 Pu fission yields have been determined by a radiochemical method. A target and a fission chamber made of same fissible material are irradied together. The total fission number is measured from the fission chamber. The fission product activities are directly measured on the target using calibrated Ge-Li detectors. The fissible material masses are determined by alpha and mass spectrometries. The irradiations were made on the critical assemblies PROSPERO and CALIBAN and on the 14 MeV neutron generator of C.E. VALDUC. 3 to 5% fission yield errors are got for the most measured nuclides: 95 Zr, 97 Zr, 99 Mo, 103 Ru, 131 I, 132 Te, 140 Ba, 141 Ce, 143 Ce, 144 Ce, 147 Nd [fr
Heavy neutron-deficient radioactive beams: fission studies and fragment distributions
Energy Technology Data Exchange (ETDEWEB)
Schmidt, K.H.; Benlliure, J.; Heinz, A.; Voss, B. [Gesellschaft fuer Schwerionenforschung mbH, Darmstadt (Germany); Boeckstiegel, C.; Grewe, A.; Steinhaeuser, S.; Clerc, H.G.; Jong, M. de; Junghans, A.R.; Mueller, J. [Technische Hochschule Darmstadt (Germany). Inst. fuer Kernphysik; Pfuetzner, M. [Warsaw Univ. (Poland). Inst. of Experimental Physics
1998-02-01
The secondary-beam facility of GSI Darmstadt was used to study the fission process of short-lived radioactive nuclei. Relativistic secondary projectiles were produced by fragmentation of a 1 A GeV {sup 238}U primary beam and identified in nuclear charge and mass number. Their production cross sections were determined, and the fission competition in the statistical deexcitation was deduced for long isotopical chains. New results on the enhancement of the nuclear level density in spherical and deformed nuclei due to collective rotational and vibrational excitations were obtained. Using these reaction products as secondary beams, the dipole giant resonance was excited by electromagnetic interactions in a secondary lead target, and fission from excitation energies around 11 MeV was induced. The fission fragments were identified in nuclear charge, and their velocity vectors were determined. Elemental yields and total kinetic energies have been determined for a number of neutron-deficient actinides and preactinides which were not accessible with conventional techniques. The characteristics of multimodal fission of nuclei around {sup 226}Th were systematically investigated and related to the influence of shell effects on the potential energy and on the level density between fission barrier and scission. A systematic view on the large number of elemental yields measured gave rise to a new interpretation of the enhanced production of even elements in nuclear fission and allowed for a new understanding of pair breaking in large-scale collective motion. (orig.)
International Nuclear Information System (INIS)
Danilyan, G. V.; Klenke, J.; Krakhotin, V. A.; Kopach, Yu. N.; Novitsky, V. V.; Pavlov, V. S.; Shatalov, P. B.
2011-01-01
Study of the T-odd three-vector correlation in the emission of prompt neutrons from 235 U fission by polarized cold neutrons has been continued at the facility MEPHISTO of the FRM II reactor (Technical University of Munich). The sought correlation was not found within experimental error of 2.3 × 10 −5 . The upper limit for the asymmetry coefficient has been set to vertical bar D n vertical bar −5 at 99% confidence level, whereas for ternary fission correlation coefficient D α = (170±20) × 10 −5 . This limit casts doubt on a model that explains the three-vector correlation in ternary fission by the Coriolis mechanism. At the same time, five-vector correlation in the emission of prompt fission neutrons has been measured, which describes the rotation of the fissioning nucleus at the moment it breaks (ROT effect). At the angle 22.5° to the fission axis, the correlation coefficient was found to be (1.57 ± 0.20) × 10 −4 , while at the angle of 67.5° it is zero within the experimental uncertainty. The existence of ROT effect in the emission of prompt fission neutrons can be explained by the anisotropy of neutron emission in the rest frame of the fragment (fission fragments are aligned with respect to the axis of deformation of the fissioning nucleus), similar to the mechanism of ROT effect in the emission of prompt γ-rays.
Energy Technology Data Exchange (ETDEWEB)
Weill, J; Duchene, J P [Commissariat a l' Energie Atomique, Saclay (France). Centre d' Etudes Nucleaires
1958-07-01
The ionisation chamber described is designed for the measurement of slow neutron fluxes of average or low intensity, in the presence, eventually, of very high gamma fluxes. The capture of a slow neutron by a fissile material, in this case {sup 235}U, gives rise to fission fragments, high-energy particles which ionise the gas contained in the chamber. The neutrons are detected by virtue of the potential pulses, on the collecting electrode of the chamber, deriving from the collection of the ions produced by the fission fragments. The pulses are counted by means of a measuring system consisting of a preamplifier, a 2 Mc amplifier, a discriminator and an electronic scale with numerator or integrator. The general characteristics are as follows: sensitivity to neutrons: 0.07 kicks/n/cm{sup 2}.s, sensitivity to {gamma} rays: zero up to 3.10{sup 4} R/H, a background noise at the normal discrimination voltage: 0.01 kicks/s, working H.T.: -500 V, capacity: 40 {mu}{mu}F, average height of pulse: 8 mV, limits of use: from several neutrons to 10{sup 6} n/cm{sup 2}.s. This chamber may be used in all cases where low fluxes of slow neutrons must be measured, especially in the presence of high gamma fluxes, for example in the checking of Pu concentrations in an extraction plant or for the starting up of reactors. (author) [French] La chambre d'ionisation decrite est destinee a la mesure des flux de neutrons lents d'intensite moyenne ou faible, en presence eventuelle de flux gamma tres importants. La capture d'un neutron lent par un materiau fissile, en l'occurrence {sup 235}U, donne naissance a des fragments de fission, particules de grande energie qui ionisent le gaz contenu dans la chambre. Les neutrons sont detectes grace aux impulsions de potentiel, sur l'electrode collectrice de la chambre, provenant de la collection des ions produits par les fragments de fission. Une chaine de mesure comprenant un preamplificateur, un amplificateur 2 Mc, un discriminateur, une echelle
International Nuclear Information System (INIS)
Tariq Siddique, M.; Kim, Myung Hyun
2014-01-01
Fusion-fission hybrid reactor can be the first milestone of fusion technology and achievable in near future. It can provide operational experience for tritium recycling for pure fusion reactor and be used for incineration of high-level long-lived waste isotopes from existing fission power reactors. Hybrid reactor for waste transmutation (Hyb-WT) was designed and optimized to assess its otential for waste transmutation. ITER will be the first large scaled experimental tokamak facility for the testing of test blanket modules (TBM) which will layout the foundation for DEMO fusion power plants. Similarly hybrid test blanket module (HTBM) will be the foundation for rationality of fusion fission hybrid reactors. Designing and testing of hybrid blankets will lead to another prospect of nuclear technology. This study is initiated with a preliminary design concept of a hybrid test blanket module (HTBM) which would be tested in ITER. The neutrons generated in D-T fusion plasma are of high energy, 14.1 MeV which could be multiplied significantly through inelastic scattering along with fission in HTBM. In current study the detailed neutronic analysis is performed for the blanket module which involves the neutron growth and loss distribution within blanket module with the choice of different fuel and coolant materials. TRU transmutation and tritium breeding performance of HTBM is analyzed under ITER irradiation environment for five different fuel types and with Li and LiPb coolants. Simple box geometry with plate type TRU fuel is adopted so that it can be modelled with heterogeneous material geometry in MCNPX. Waste transmutation ratio (WTR) of TRUs and tritium breeding ration (TBR) is computed to quantify the HTBM performance. Neutron balance is computed in detail to analyze the performance parameters of HTBM. Neutron spectrum and fission to capture ratio in TRU fuel types is also calculated for detailed analysis of HTBM
Energy Technology Data Exchange (ETDEWEB)
Tariq Siddique, M.; Kim, Myung Hyun [Kyung Hee Univ., Yongin (Korea, Republic of)
2014-05-15
Fusion-fission hybrid reactor can be the first milestone of fusion technology and achievable in near future. It can provide operational experience for tritium recycling for pure fusion reactor and be used for incineration of high-level long-lived waste isotopes from existing fission power reactors. Hybrid reactor for waste transmutation (Hyb-WT) was designed and optimized to assess its otential for waste transmutation. ITER will be the first large scaled experimental tokamak facility for the testing of test blanket modules (TBM) which will layout the foundation for DEMO fusion power plants. Similarly hybrid test blanket module (HTBM) will be the foundation for rationality of fusion fission hybrid reactors. Designing and testing of hybrid blankets will lead to another prospect of nuclear technology. This study is initiated with a preliminary design concept of a hybrid test blanket module (HTBM) which would be tested in ITER. The neutrons generated in D-T fusion plasma are of high energy, 14.1 MeV which could be multiplied significantly through inelastic scattering along with fission in HTBM. In current study the detailed neutronic analysis is performed for the blanket module which involves the neutron growth and loss distribution within blanket module with the choice of different fuel and coolant materials. TRU transmutation and tritium breeding performance of HTBM is analyzed under ITER irradiation environment for five different fuel types and with Li and LiPb coolants. Simple box geometry with plate type TRU fuel is adopted so that it can be modelled with heterogeneous material geometry in MCNPX. Waste transmutation ratio (WTR) of TRUs and tritium breeding ration (TBR) is computed to quantify the HTBM performance. Neutron balance is computed in detail to analyze the performance parameters of HTBM. Neutron spectrum and fission to capture ratio in TRU fuel types is also calculated for detailed analysis of HTBM.
A search for back-to-back e+e- pairs in the spontaneous-fission disintegration of 252Cf
International Nuclear Information System (INIS)
Tsunoda, T.; Nakamura, S.; Orito, S.; Minowa, M.
1995-01-01
A back-to-back electron-positron pair is searched for in spontaneous-fission disintegration of 252 Cf. The emission of such a pair, if observed, might be a manifestation of production and prompt decay of a heretofore unknown neutral particle. The emission rate of such a pair is found to be less than (2.5-5.5) . 10 -10 per fission at the 95% confidence level depending on the mass of the hypothetical particle which is between 40 and 200 MeV/c 2 . (orig.)
International Nuclear Information System (INIS)
Bertalot, L.
1987-01-01
A feasibility study has been carried out on the use of in-core fission chambers as neutron diagnostic tools to perform neutron flux measurements on the blanket component of NET. The high neutron and gamma fluxes and the severe thermal-mechanical and magnetic conditions of the blanket structure have been taken into account in this analysis. Preliminary design criteria and specifications of an in-core detector are presented for NET application. A research and development programme is outlined which aims to obtain more information on the tecnological constraints arising from the severe conditions of the NET blanket
Effects of fission neutrons and X-rays on the epithelium of the mouse stomach
International Nuclear Information System (INIS)
Kingma-ter Haar, J.M.
1982-07-01
A quantitative study is presented of the effects of whole-body irradiation on the stomach of mice. Two types of ionizing radiation were compared - fast fission neutrons of 1.0 MeV mean energy and 300 kVp X-rays. The effects on the functional cell populations, on gastric secretion and on gastric stem cell populations were studied. These effects have been investigated a) for a neutron dose in the lethal dose-range of 4.0 Gy as a function of time and b) at a post-irradiation interval of 3 weeks as a function of neutron and X-ray dose. (Auth.)
Approaches for the generation of a covariance matrix for the Cf-252 fission-neutron spectrum
International Nuclear Information System (INIS)
Mannhart, W.
1983-01-01
After a brief retrospective glance is cast at the situation, the evaluation of the Cf-252 neutron spectrum with a complete covariance matrix based on the results of integral experiments is proposed. The different steps already taken in such an evaluation and work in progress are reviewed. It is shown that special attention should be given to the normalization of the neutron spectrum which must be reflected in the covariance matrix. The result of the least-squares adjustment procedure applied can easily be combined with the results of direct spectrum measurements and should be regarded as the first step in a new evaluation of the Cf-252 fission-neutron spectrum. (author)
International Nuclear Information System (INIS)
Broerse, J.J.; Bekkum, D.W. van; Hollander, C.F.; Davids, J.A.G.
1978-01-01
In order to assess the risk of exposure to ionizing radiation in man, and to evaluate the results of therapeutic measures, the mortality of rhesus monkeys irradiated with X-rays and fission neutrons and the effect of autologous bone marrow transplantation have been investigated. The LDsub(50/30d) values for X- and neutron-irradiated monkeys amount to 525 and 260 rad respectively, resulting in an r.b.e. of approximately 2 for the occurrence of the bone marrow syndrome. Protection of the animals by autologous bone marrow transplantation was observed up to doses of 860 rad of X-rays and 440 rad of fission neutrons. After both fission-neutron irradiation and X-irradiation in the lowest range of lethal doses, the bone marrow syndrome was found to occur without the concurrent incidence of the intestinal syndrome. The studies indicate that, for humans accidentally exposed to what would otherwise be lethal doses of fast neutrons, bone marrow transplantation may be beneficial. (author)
Technique of neutron-induced (fission-track) autoradiography with histological detail
International Nuclear Information System (INIS)
Smith, J.M.; Taylor, G.N.; Jee, W.S.S.
1980-01-01
The primary advantage of neutron-induced or fission-track autoradiography compared with conventional autoradiography is that for low concentrations of fissile nuclides prohibitively long exposure times may be avoided. However, it is difficult to produce imaging of biological structures on the neutron-induced autoradiograph which would allow localization of the nuclide histologically. The technique presented circumvents this difficulty using a thin polycarbonate film applied to the histologically stained tissue section mounted on a quartz substrate. After irradiation of the tissue section with an appropriate thermal neutron flux, the fission fragment tracks are revealed by etching the film with KOH. The tracks, superimposed on the stained tissue, may be observed under the light microscope in the same manner as for conventional nuclear emulsion autoradiography
Multi-fold correlations between 252Cf (sf) fragments and fission neutrons/γ-rays
International Nuclear Information System (INIS)
Duering, I.; Jahnke, U.
1993-01-01
Direction-sensitive spectroscopy of fission fragments (twin ionization chamber with Frisch grids) was combined with the measurement of neutron multiplicity distribution (P(ν), average total γ-ray energy (2x2 π Gd-loaded scintillator) as well as energy and angular distribution of neutrons and γ-rays. Based on the careful account for necessary corrections, scission configurations given by mass asymmetry, elongation (total kinetic energy of fragments), and shape asymmetry (ν 1 /ν 2 ) can be studied exclusively in correlation with differential distributions of emission products. The scheme for correcting the neutron multiplicity distribution including its separation into the contributions from the complementary fragments is presented in detail. The mass yield for extreme anti ν 1 / anti ν 2 ratios show fine structures indicating the cold shape-asymmetric fission. (orig.)
Evaluation of secondary and prompt fission neutron spectra
Energy Technology Data Exchange (ETDEWEB)
Porodzinskij, Yu.V.; Sukhovitskij, E.Sh. [Radiation Physics and Chemistry Problems Inst., Minsk-Sosny (Belarus)
1997-03-01
A simple model allowing to split neutron emission spectra into reaction partials is suggested. Predicted spectra of (n,n`{gamma}), (n,n`f), etc appear to be much harder than usually evaluated. (author)
Realistic fission models, new beta-decay half-lives and the r-process in neutron star mergers
International Nuclear Information System (INIS)
Shibagaki, S.; Kajino, T.; Chiba, S.; Lorusso, G.; Nishimura, S.; Mathews, G. J.
2014-01-01
Almost half of heavy nuclei beyond iron are considered to be produced by rapid neutron capture process (r-process). This process occurs in the neutron-rich environment such as core-collapse supernovae or neutron star mergers, but the main production site is still unknown. In the r-process of neutron star mergers, nuclear fission reactions play an important role. Also beta-decay half-lives of magic nuclei are crucial for the r-process. We have carried out r-process nucleosynthesis calculations based upon new theoretical estimates of fission fragment distributions and new beta-decay half-lives for N=82 nuclei measured at RIBF-RIKEN. We investigate the effect of nuclear fission on abundance patterns in the matter ejected from neutron star mergers with two different fission fragment mass distributions. We also discuss how the new experimental beta-decay half-lives affect the r-process
Monte carlo sampling of fission multiplicity.
Energy Technology Data Exchange (ETDEWEB)
Hendricks, J. S. (John S.)
2004-01-01
Two new methods have been developed for fission multiplicity modeling in Monte Carlo calculations. The traditional method of sampling neutron multiplicity from fission is to sample the number of neutrons above or below the average. For example, if there are 2.7 neutrons per fission, three would be chosen 70% of the time and two would be chosen 30% of the time. For many applications, particularly {sup 3}He coincidence counting, a better estimate of the true number of neutrons per fission is required. Generally, this number is estimated by sampling a Gaussian distribution about the average. However, because the tail of the Gaussian distribution is negative and negative neutrons cannot be produced, a slight positive bias can be found in the average value. For criticality calculations, the result of rejecting the negative neutrons is an increase in k{sub eff} of 0.1% in some cases. For spontaneous fission, where the average number of neutrons emitted from fission is low, the error also can be unacceptably large. If the Gaussian width approaches the average number of fissions, 10% too many fission neutrons are produced by not treating the negative Gaussian tail adequately. The first method to treat the Gaussian tail is to determine a correction offset, which then is subtracted from all sampled values of the number of neutrons produced. This offset depends on the average value for any given fission at any energy and must be computed efficiently at each fission from the non-integrable error function. The second method is to determine a corrected zero point so that all neutrons sampled between zero and the corrected zero point are killed to compensate for the negative Gaussian tail bias. Again, the zero point must be computed efficiently at each fission. Both methods give excellent results with a negligible computing time penalty. It is now possible to include the full effects of fission multiplicity without the negative Gaussian tail bias.
Neutron-induced fission fragment angular distribution at CERN n TOF: The Th-232 case
Tarrio, Diego; Paradela, Carlos
This thesis work was done in the frame of the study of the neutron-induced fission of actinides and subactinides at the CERN n TOF facility using a fast Parallel Plate Avalanche Counters (PPACs) setup. This experimental setup provide us with an intense neutron beam with a white spectrum from thermal to 1 GeV and with an outstanding high resolution provided by its flight path of 185 m. In our experiment, fission events were identified by detection of both fission fragments in time coincidence in the two PPAC detectors flanking the corresponding target. This technique allowed us to discriminate the fission events from the background produced by α disintegration of radioactive samples and by particles produced in spallation reactions. Because PPAC detectors are insensitive to the γ flash, it is possible to reach energies as high as 1 GeV. The stripped cathodes provide the spatial position of the hits in the detectors, so that the emission angle of the fission fragments can be measured. Inside the reaction cham...
International Nuclear Information System (INIS)
Carlsson, Magnus
2004-06-01
Areas ranging from nuclear structure models to accelerator-driven systems benefit from improved neutron-induced fission data in the intermediate energy region. In this Master's degree thesis, the fragment angular distribution from fission of 238 U, induced by 21-MeV neutrons, has been analysed from an experiment performed with the Medley/DIFFICILE setup at the The Svedberg Laboratory in Uppsala. The data have been corrected for low energy neutrons in the beam. The results agree with other experiments, as well as with model calculations. The data should be a starting point for further analysis with a goal to deduce the fission cross-section of 238 U
A search for fine structure of the time-of-flight spectrum of the fission neutrons of 252Cf
International Nuclear Information System (INIS)
Scobie, J.; Scott, R.D.; Feather, N.; Vass, D.G.
1977-01-01
A standard time-of-flight arrangement, in which start pulses were supplied by fission fragments and stop pulses by neutrons, has been employed in an attempt to check recent claims of the existence of fine structures in the time-of-flight spectrum of the fission neutrons of 252 Cf. This structure, in the form of spikes with tails towards longer times, has been attributed to the emission of neutrons of short delay (with half-lives of a few to a hundred or so nanoseconds) in the fission process. It has not been possible to find any convincing evidence for the existence of such structure. (author)
International Nuclear Information System (INIS)
Perez, R.B.; Difilippo, F.C.; Saussure, G. de; Ingle, R.W.
1978-01-01
A measurement of the 238 U fission cross section between 5 eV and 3.5 MeV was performed. Included is the identification of 85 resonances or clusters of resonances below 200 keV. Also the fission widths for the 27 resolved class I levels were computed from their fission areas, and a neutron width of 0.005 MeV was estimated for the quasi-class II level in the 721 eV fission cluster. The fission level spacing and cross sections are discussed. 9 references
Danilyan, G V; Pavlov, V S; Fedorov, A V
2001-01-01
The results of the experiment for the search of the sp-interference effect in the distribution of the prompt neutrons of the sup 2 sup 3 sup 5 U fission by thermal polarized neutrons are presented. The experiment is carried out on the polarized neutrons beam of the MIFI reactor. The scheme of the installation and the flight time spectrum are presented
Possible viscosity effects in neutron-induced fission of 232Th and 238U
International Nuclear Information System (INIS)
Gindler, J.E.; Glendenin, L.E.; Wilkins, B.D.
1979-01-01
Fission yields induced in the 238 U(n,f) and 232 Th(n,f) reactions were determined as a function of incident neutron energy (E/sub n/). The ratio of 115 Cd-to- 140 Ba yields as a function of E/sub n/ is analyzed by means of the equation Y 1 /Y 2 = exp[2(a 1 (E/sub n/+E 1 )/sup 1/2/ -2(a 2 (E/sub n/+E 2 )/sup 1/2/] to give values of a/sub i/, the level density parameter, and E/sub i/, the excitation energy for E/sub n/=0. The energies E/sub i/ are interpreted on the basis of the liquid drop model with shell and pairing corrections. Values are deduced for the energy dissipated by viscosity effects in the descent from the saddle point to the point where masses are fixed in the fissioning nucleus. These values are 1.7 MeV for 232 Th(n,f) and 4.8 MeV for 238 U(n,f). These values are consistent with the experimental observation that anti ν/sub p/ is approx. 0.6 neutron greater for 239 U fission than for 233 Th fission and that strong odd--even (nucleon pairing) effects are found in the fragment total kinetic energy distribution for 230 Th fission but not for 234 U fission. The low dissipation energy values together with the low values of pre-scission kinetic energy deduced by Guet, et al., [Nucl. Phys. A134 (1971)1] indicate a shorter path from the saddle point of the fissioning nucleus to scission than is generally assumed in theoretical calculations. 31 references
Beta decay heat following U-235, U-238 and Pu-239 neutron fission
Li, Shengjie
1997-09-01
This is an experimental study of beta-particle decay heat from 235U, 239Pu and 238U aggregate fission products over delay times 0.4-40,000 seconds. The experimental results below 2s for 235U and 239Pu, and below 20s for 238U, are the first such results reported. The experiments were conducted at the UMASS Lowell 5.5-MV Van de Graaff accelerator and 1-MW swimming-pool research reactor. Thermalized neutrons from the 7Li(p,n)7Be reaction induced fission in 238U and 239Pu, and fast neutrons produced in the reactor initiated fission in 238U. A helium-jet/tape-transport system rapidly transferred fission fragments from a fission chamber to a low background counting area. Delay times after fission were selected by varying the tape speed or the position of the spray point relative to the beta spectrometer that employed a thin-scintillator-disk gating technique to separate beta-particles from accompanying gamma-rays. Beta and gamma sources were both used in energy calibration. Based on low-energy(energies 0-10 MeV. Measured beta spectra were unfolded for their energy distributions by the program FERD, and then compared to other measurements and summation calculations based on ENDF/B-VI fission-product data performed on the LANL Cray computer. Measurements of the beta activity as a function of decay time furnished a relative normalization. Results for the beta decay heat are presented and compared with other experimental data and the summation calculations.
Neutron-induced fission cross sections of uraniums up to 40 MeV
Energy Technology Data Exchange (ETDEWEB)
Maslov, V.M. [Radiation Physics and Chemistry Problems Inst., Minsk-Sosny (Belarus); Hasegawa, A.
1998-11-01
Statistical theory of nuclear reactions, well-proved below 20 MeV, is applied for {sup 235}U and {sup 238}U fission data analysis up to {approx}40 MeV. It is shown that measured data could be reproduced. Chance structure of measured fission cross section is provided, it`s validity is supported by description of data for competing (n,xn)-reactions. Role of fissility of target nucleus is addressed. It seems that gap in incident neutron energy interval of 20 MeV - 50 MeV, below which evaluation approaches are well-developed, and above which simplified statistical approaches are valid, could be covered. (author)
Determination of the average number of neutrons per fission event for californium-252
International Nuclear Information System (INIS)
Aleksandrov, B.M.; Belov, L.M.; Drapchinskij, L.V.
1982-01-01
By means of a separate determination of neutron yields and fission event rates, the value of #betta#-bar( 252 Cf) has been measured for a series of new high-purity sources. The improved quality of the source active layers has reduced the error in determining the fission rate to 0.35%. The value obtained for #betta#-bar( 252 Cf) is 3.747+-0.036. A description is given of the design and the parameters of a spherical manganese bath in which the work on refining the value of #betta#-bar( 252 Cf) will be continued. (author)
Simulation of neutron rich nuclei production through 239U fission at intermediates energies
International Nuclear Information System (INIS)
Mirea, M.; Clapier, F.; Pauwels, N.; Proust, J.
1997-01-01
The theoretical part and some results obtained from a model realised for fission processes in wide range of mass-asymmetries are presented. The fission barriers are computed in a tridimensional configuration space using the Yukawa - plus - exponential macroscopic energies corrected within the Strutinsky procedure. It is assumed that channel probabilities are proportional with Gamow penetrabilities. The model is applied for the disintegration of the 239 U in order to determine the relative yields for the production of neutron rich nuclei at diverse intermediate energies. (author)
International Nuclear Information System (INIS)
Behrens, J.W.
1977-01-01
Recent studies have shown straightforward systematic behavior as a function of constant proton and neutron number for neutron-induced fission cross sections of the actinide elements in the incident-neutron energy range 3 to 5 MeV. In this report, the second in a series, fission cross-section values are studied over the MeV incident-neutron energy range, and at 0.0253 eV. Fission-barrier heights and neutron-binding energies are correlated by constant proton and neutron number; however, these systematic behaviors alone do not explain the trends observed in the fission cross-section values
Evaluating the 239Pu Prompt Fission Neutron Spectrum Induced by Thermal to 30 MeV Neutrons
Directory of Open Access Journals (Sweden)
Neudecker D.
2016-01-01
Full Text Available We present a new evaluation of the 239Pu prompt fission neutron spectrum (PFNS induced by thermal to 30 MeV neutrons. Compared to the ENDF/B-VII.1 evaluation, this one includes recently published experimental data as well as an improved and extended model description to predict PFNS. For instance, the pre-equilibrium neutron emission component to the PFNS is considered and the incident energy dependence of model parameters is parametrized more realistically. Experimental and model parameter uncertainties and covariances are estimated in detail. Also, evaluated covariances are provided between all PFNS at different incident neutron energies. Selected evaluation results and first benchmark calculations using this evaluation are briefly discussed.
Lantz, M; Al-Adili, A; Jokinen, A; Kolhinen, V; Mattera, A; Rinta-Antila, S; Penttilä, H; Pomp, S; Rakoupoulos, V; Simutkin, V; Solders, A
2014-01-01
The ERINDA funded scientific visit has enabled the groups at U ppsala Uni- versity and University of Jyväskylä to work closer together on the design of a neutron converter that will be used as neutron source in fissi on yield studies at the IGISOL-JYFLTRAP facility at the University of Jyväsk ylä. The design is based on simulations with both deterministic codes and Mo nte Carlo codes, and an ERINDA funded benchmark measurement. In order to obta in a com- petitive count rate the fission targets will be placed very cl ose to the neutron converter. The intention is to have a flexible design that wil l enable neutron fields with different energy distributions. In this report t he progression and the present status of the design work will be discussed, togethe r with an outlook of the future plans
Nuclear data requirements for fission reactor neutronics calculations
International Nuclear Information System (INIS)
Finck, P.
1998-01-01
The paper discusses current European nuclear data measurement and evaluation requirements for fission reactor technology applications and problems involved in meeting the requirements. Reference is made to the NEA High Priority Nuclear Data Request List and to the production of the new JEFF-3 library of evaluated nuclear data. There are requirements for both differential (or basic) nuclear data measurements and for different types of integral measurement critical facility measurements and isotopic sample irradiation measurements. Cross-section adjustment procedures are being used to take into account the simpler types of integral measurement, and to define accuracy needs for evaluated nuclear data
International Nuclear Information System (INIS)
Merriman, L.D.
1984-04-01
Cumulative fission-product yields have been determined for 13 gamma rays emitted during the decay of 12 fission products created by thermal-neutron fission of 243 Cm. A high-resolution low-energy germanium detector was used to measure the pulse-height spectra of gamma rays emitted from a 77-nanogram sample of 243 Cm after the sample had been irradiated by thermal neutrons. Analysis of the data resulted in the identification and matching of gamma-ray energies and half-lives to individual radioisotopes. From these results, 12 cumulative fission product yields were deduced for radionuclides with half-lives between 4.2 min and 84.2 min. 7 references
International Nuclear Information System (INIS)
Armelin, M.J.A.
1984-01-01
A system for the detection and counting of delayed neutrons which allows the analysis of some fissile and fertile nuclides, in samples of milligram size, was developed. This was applied for the analysis of natural uranium and thorium and also for determining the 235 U/ 238 U ratio in non-irradiated samples which contain uranium with different degrees of enrichment in 235 U. The spectrum of activated neutrons was varied in order to discriminate the nuclides, by covering or not the sample with a material (cadmium or boron) able to absorb low energy neutrons. Determination of 235 U/ 238 U ratios, through the number of delayed neutrons, was made by drawing a calibration curve using standards ranging from 0.5% to 93% on 235 U; the accuracy of the method was also examined. In a first step, conditions for a simultaneous and non-destructive analysis of uranium and thorium were developed. The interference between these two nuclides was studied, using simulated samples. Real samples were provided by Nuclemon and IAEA. For samples with uranium concentration in the range of percentages and thorium concentration of some ppm, uranium interferes in the determination of thorium through the non-destructive analytical method. For this case, a fast and quantitative chemical method was studied which allows for the separation of thorium from uranium before the determination of throrium concentration by counting the delayed fission neutrons. It was found that the results obtained by both destructive and non-destructive methods are very consistent and can be considered statistically equivalent within a confidence level of 95%. (Author) [pt
Directory of Open Access Journals (Sweden)
Mounia Laassiri
Full Text Available For efficient exploitation of research reactors, it is important to discern neutron flux distribution inside the reactor with the best possible precision. For this reason, fission and ionization chambers are used to measure the neutron field. In these arrays, the sequences of the neutron interaction points in the fission chamber can correctly be identified in order to obtain true neutron energies emitted by nuclei of interest. However, together with the neutrons, gamma-rays are also emitted from nuclei and thereby affect neutron spectra. The originality of this study consists in the application of tensor based blind source separation methods to extract independent components from signals recorded at the fission chamber preamplifier’s output. The objective is to achieve software neutron-gamma discrimination using Nonnegative Tensor Factorization tools. For reasons of nuclear safety, we first simulate the neutron flux inside the TRIGA Mark II Reactor using Monte Carlo methods under Geant4 platform linked to Garfield++. Geant4 simulations allow the fission chamber construction whereas linking the model to Garfield++ permits to simulate drift parameters from the ionization of the filling gas, which is not possible otherwise. Keywords: Fission chamber (FC, Geant4, Garfield++, Neutron-gamma discrimination, Nonnegative Tensor Factorization (NTF
Development of a position-sensitive fission counter and measurement of neutron flux distributions
International Nuclear Information System (INIS)
Yamagishi, Hideshi; Soyama, Kazuhiko; Kakuta, Tsunemi
2001-08-01
A position-sensitive fission counter (PSFC) that operates in high neutron flux and high gamma-ray background such as at the side of a power reactor vessel has been developed. Neutron detection using the PSFC with a solenoid electrode is based on a delay-line method. The PSFC that has the outer diameter of 25 mm and the sensitive length of 1000 mm was manufactured for investigation of the performances. The PSFC provided output current pulses that were sufficiently higher than the alpha noise, though the PSFC has a solenoid electrode and large electrode-capacitance. The S/N ratio of PSFC outputs proved to be higher than that of ordinary fission counters with 200 mm sensitive length. A performance test to measure neutron flux distributions by a neutron measuring system with the PSFC was carried out by the side of a graphite pile, W2.4 x H1.4 x L1.2 m, with neutron sources, Am-Be 370 GBq x 2. It was confirmed that the neutron flux distribution was well measured with the system. (author)
Monitoring the fast neutrons in a high flux: The case for 242Pu fission chambers
International Nuclear Information System (INIS)
Filliatre, P.; Jammes, C.; Oriol, L.; Geslot, B.; Vermeeren, L.
2009-01-01
Fission chambers are widely used for on-line monitoring of neutron fluxes in irradiation reactors. A selective measurement of a component of interest of the neutron flux is possible in principle thanks to a careful choice of the deposit material. However, measuring the fast component is challenging when the flux is high (up to 10 15 n/cm 2 /s) with a significant thermal component. The main problem is that the isotopic content of a material selected for its good response to fast neutrons evolves with irradiation, so that the material is more and more sensitive to thermal neutrons. Within the framework of the FNDS (Fast Neutron Detector System) project, we design tools that simulate the evolution of the isotopic composition and fission rate for several deposits under any given flux. In the case of a high flux with a significant thermal component, 242 Pu is shown after a comprehensive study of all possibilities to be the best choice for measuring the fast component, as long as its purity is sufficient. If an estimate of the thermal flux is independently available, one can correct the signal for that component. This suggests a system of two detectors, one of which being used for such a correction. It is of very high interest when the detectors must be operated up to a high neutron fluence. (authors)
Monitoring the fast neutrons in a high flux: The case for {sup 242}Pu fission chambers
Energy Technology Data Exchange (ETDEWEB)
Filliatre, P.; Jammes, C.; Oriol, L.; Geslot, B. [Commissariat a l' Energie Atomique, DEN/SPEX/LDCI, Centre de Cadarache, F-13108 Saint-Paul-lez-Durance (France); Vermeeren, L. [SCK-CEN, Boeretang 200, B-2400 Mol (Belgium)
2009-07-01
Fission chambers are widely used for on-line monitoring of neutron fluxes in irradiation reactors. A selective measurement of a component of interest of the neutron flux is possible in principle thanks to a careful choice of the deposit material. However, measuring the fast component is challenging when the flux is high (up to 10{sup 15} n/cm{sup 2}/s) with a significant thermal component. The main problem is that the isotopic content of a material selected for its good response to fast neutrons evolves with irradiation, so that the material is more and more sensitive to thermal neutrons. Within the framework of the FNDS (Fast Neutron Detector System) project, we design tools that simulate the evolution of the isotopic composition and fission rate for several deposits under any given flux. In the case of a high flux with a significant thermal component, {sup 242}Pu is shown after a comprehensive study of all possibilities to be the best choice for measuring the fast component, as long as its purity is sufficient. If an estimate of the thermal flux is independently available, one can correct the signal for that component. This suggests a system of two detectors, one of which being used for such a correction. It is of very high interest when the detectors must be operated up to a high neutron fluence. (authors)
Fission ionisation chamber for the measurement of low fluxes of slow neutrons
International Nuclear Information System (INIS)
Weill, J.; Duchene, J.P.
1958-01-01
The ionisation chamber described is designed for the measurement of slow neutron fluxes of average or low intensity, in the presence, eventually, of very high gamma fluxes. The capture of a slow neutron by a fissile material, in this case 235 U, gives rise to fission fragments, high-energy particles which ionise the gas contained in the chamber. The neutrons are detected by virtue of the potential pulses, on the collecting electrode of the chamber, deriving from the collection of the ions produced by the fission fragments. The pulses are counted by means of a measuring system consisting of a preamplifier, a 2 Mc amplifier, a discriminator and an electronic scale with numerator or integrator. The general characteristics are as follows: sensitivity to neutrons: 0.07 kicks/n/cm 2 .s, sensitivity to γ rays: zero up to 3.10 4 R/H, a background noise at the normal discrimination voltage: 0.01 kicks/s, working H.T.: -500 V, capacity: 40 μμF, average height of pulse: 8 mV, limits of use: from several neutrons to 10 6 n/cm 2 .s. This chamber may be used in all cases where low fluxes of slow neutrons must be measured, especially in the presence of high gamma fluxes, for example in the checking of Pu concentrations in an extraction plant or for the starting up of reactors. (author) [fr
Assay of fissionable isotopes in aqueous solution by pulsed neutron interrogation
International Nuclear Information System (INIS)
Campbell, P.; Gardy, E.M.; Boase, D.G.
1978-04-01
Non-destructive assay of uranium-235 and thorium-232 in aqueous nitric acid solutions has been accomplished by irradiation with pulses of neutrons from a 14-MeV Cockcroft-Walton neutron generator, and counting of the delayed neutrons emitted from the fissions induced. Design of the delayed neutron detector assemblies is described, together with the neutron pulse timing and counting systems. The effects of irradiation time, counting time, neutron moderation, detector design and sample geometry on the delayed neutron response from uranium-235 and 238 and thorium-232 are discussed. By using polyethylene to moderate the interrogating neutrons, solutions can be analyzed for both uranium-235 and thorium. Comparative analyses with chemical and γ-spectrometric methods show good agreement. The neutron method is rapid and is shown to be unaffected by the presence in solution of impurities such as iron, nickel, chromium, and aluminum. With the experimental equipment described, detection limits of 0.6 mg of 235 U and 9 mg of 232 Th in a sample volume of 25 mL have been achieved. Analyses of highly radioactive samples may be done easily since the measurements are not affected by the presence of large amounts of βγ radiation. Samples can be enclosed in small lead-shielded flasks during analysis to protect the analyst. The potential of the technique to on-line analysis applications is explored briefly. (author)
International Nuclear Information System (INIS)
Barnard, R.W.; Jensen, D.H.
1982-01-01
Uranium formations are assayed by prompt fission neutron logging techniques. The uranium in the formation is proportional to the ratio of epithermal counts to thermal or eqithermal dieaway. Various calibration factors enhance the accuracy of the measurement
Observation of new spontaneous fission activities from elements 100 to 105
International Nuclear Information System (INIS)
Somerville, L.P.
1982-03-01
Several new Spontaneous Fission (SF) activities have been found. No definite identification could be made for any of the new SF activities; however, half-lives and possible assignments to element-104 isotopes consistent with several cross bombardments include 257 Rf(3.8 s, 14% SF), 258 Rf(13 ms), 259 Rf(approx. 3 s, 8% SF), 260 Rf(approx. 20 ms), and 262 Rf(approx. 50 ms). The 80-ms SF activity claimed by the Dubna group for the discovery of element 104 ( 260 104) was not observed. A difficulty exists in the interpretation that 260 Rf is a approx. 20-ms SF activity: in order to be correct, for example, the SF activities with half-lives between 14 and 24 ms produced in the reactions 109- to 119-MeV 18 O + 248 Cm, 88- to 100-MeV 15 N + 249 Bk, and 96-MeV 18 O + 249 Cf must be other nuclides due to their large production cross sections, or the cross sections for production of 260 Rf must be enhanced by unknown mechanisms. Based on calculated total production cross sections a possible approx. 1% electron-capture branch in 258 Lr(4.5 s) to the SF emitter 258 No(1.2 ms) and an upper limit of 0.05% for SF branching in 254 No(55 s) were determined. Other measured half-lives from unknown nuclides produced in respective reactions include approx. 1.6 s ( 18 O + 248 CM), indications of a approx. 47-s SF activity (75-MeV 12 C + 249 Cf), and two or more SF activities with 3 s less than or equal to T/sub 1/2/ less than or equal to 60 s ( 18 O + 249 Bk). The most exciting conclusion of this work is that if the tentative assignments to even-even element 104 isotopes are correct, there would be a sudden change in the SF half-life systematics at element 104 which has been predicted theoretically and attributed to the disappearance of the second hump of the double-humped fission barrier
Energy Technology Data Exchange (ETDEWEB)
Goverdovski, A.A.; Khryachkov, V.A.; Ketlerov, V.V.; Mitrofanov, V.F.; Ostapenko, Yu.B.; Semenova, N.N.; Fomichev, A.N.; Rodina, L.F. [Institute of Physics and Power Engineering, Obninsk (Russian Federation)
1997-03-01
Twin gridded ionization chamber and corresponding software was designed for measurements of masses, kinetic energies and nuclear charges of fission fragments from fast neutron induced fission of {sup 237}Np. The ionization detector design, electronics, data acquisition and processing system and the test results are presented in this paper. (J.P.N.)
Koltick, D.; McConchie, S.; Sword, E.
2008-04-01
The design and performance of a pulseable neutron source utilizing a D-T neutron generator and a depleted uranium reflector are presented. Approximately half the generator's 14 MeV neutron flux is used to produce a fission-like neutron spectrum similar to 252Cf. For every 14 MeV neutron entering the reflector, more than one fission-like neutron is reflected back across the surface of the reflector. Because delayed neutron production is more than two orders of magnitude below the prompt neutron production, the source takes full advantage of the generator's pulsed mode capability. Applications include all elemental characterization systems using neutron-induced gamma-ray spectroscopy. The source simultaneously emits 14 MeV neutrons optimal to excite fast neutron-induced gamma-ray signals, such as from carbon and oxygen, and fission-like neutrons optimal to induce neutron capture gamma-ray signals, such as from hydrogen, nitrogen, and chlorine. Experiments were performed, which compare well to Monte Carlo simulations, showing that the uranium reflector enhances capture signals by up to a factor of 15 compared to the absence of a reflector.
International Nuclear Information System (INIS)
Gwin, R.; Spencer, R.R.; Ingle, R.W.; Todd, J.H.; Weaver, H.
1980-01-01
The average number of prompt neutrons emitted per fission ν/sub p/-bar(E), was measured for 235 U relative to ν/sub p/-bar for the spontaneous fission of 252 Cf over the neutron energy range from 500 eV to 10 MeV. The samples of 235 U and 252 Cf were contained in fission chambers located in the center of a large liquid scintillator. Fission neutrons were detected by the large liquid scintillator. The present values of ν/sub p/-bar(E) for 235 U are about 0.8% larger than those measured by Boldeman. In earlier work with the present system, it was noted that Boldeman's value of ν/sub p/-bar(E) for thermal energy neutrons was about 0.8% lower than obtained at ORELA. It is suggested that the thickness of the fission foil used in Boldeman's experiment may cause some of the discrepancy between his and the present values of ν/sub p/-bar(E). For the energy region up to 700 keV, the present values of ν/sub p/-bar(E) for 235 U agree, within the uncertainty, with those given in ENDF/B-V. Above 1 MeV the present results for ν/sub p/-bar(E) range about the ENDF/B-V values with differences up to 1.3%. 6 figures, 1 table
Performance test of micro-fission chambers for in-vessel neutron monitoring of ITER
International Nuclear Information System (INIS)
Yamauchi, Michinori; Nishitani, Takeo; Ochiai, Kentaro; Morimoto, Yuichi; Hori, Jun-ichi; Ebisawa, Katsuyuki; Kasai, Satoshi
2002-03-01
A micro-fission chamber with 12 mg UO 2 and a dummy chamber without uranium were fabricated and the performance was tested. They are designed to be installed inside the vacuum vessel of the compact ITER (ITER-FEAT) for neutron monitoring. The vacuum leak rate of the dummy chamber with MI cable, resistances of chambers between central conductor and outer sheath, and mechanical strength up to 50G acceleration were confirmed to meet the design criteria. The gamma-ray sensitivity was measured for the dummy chamber with the 60 Co gamma-ray irradiation facility at JAERI Takasaki. The output signals for gamma-rays in Campbelling mode were estimated to be less than 0.1% of those by neutrons at the location behind the blanket module in ITER-FEAT. The detector response for 14 MeV neutrons was investigated with the FNS facility. Excellent linearity between count rates, square of Campbelling voltage and neutron fluxes was confirmed in the temperature range from 20degC (room) to 250degC. However, a positive dependence of 14 MeV neutron count rates on temperature was observed, which might be caused by the increase in the pulse height with temperature rise. Effects of a change of surrounding materials were evaluated by the sensitivity measurements of the micro-fission chamber inserted into the shielding blanket mock-up. The sensitivity was enhanced by slow-downed neutrons, which agreed with the calculation result by MCNP-4C code. As a result, it was concluded that the developed micro-fission chamber is applicable for ITER-FEAT. (author)
A proton-driven, intense, subcritical, fission neutron source for radioisotope production
Energy Technology Data Exchange (ETDEWEB)
Jongen, Y. [Chemin du Cyclotron, Louvain-la-Neuve (Belgium)
1995-10-01
{sup 99m}Tc, the most frequently used radioisotope in nuclear medicine, is distributed as {sup 99}Mo=>{sup 99m}Tc generators. {sup 99}Mo is a fission product of {sup 235}U. To replace the aging nuclear reactors used today for this production, the author proposes to use a spallation neutron source, with neutron multiplication by fission. A 150 MeV, H{sup {minus}} cyclotron can produce a 225 kW proton beam with 50% total system energy efficiency. The proton beam would hit a molten lead target, surrounded by a water moderator and a graphite reflector, producing around 0.96 primary neutron per proton. The primary spallation neutrons, moderated, would strike secondary targets containing a subcritical amount of {sup 235}U. The assembly would show a k{sub eff} of 0.8, yielding a fivefold neutron multiplication. The thermal neutron flux at the targets location would be 2 {times} 10{sup 14} n/cm{sup 2}.s, resulting in a fission power of 500 to 750 kW. One such system could supply the world demand in {sup 99}Mo, as well as other radioisotopes. Preliminary indications show that the cost would be lower than the cost of a commercial 10 MW isotope production reactor. The cost of operation, of disposal of radiowaste and of decommissioning should be significantly lower as well. Finally, the non-critical nature of the system would make it more acceptable for the public than a nuclear reactor and should simplify the licensing process.
238U neutron-induced fission cross section for incident neutron energies between 5 eV and 3.5 MeV
International Nuclear Information System (INIS)
Difilippo, F.C.; Perez, R.B.; de Saussure, G.; Olsen, D.K.; Ingle, R.W.
1979-01-01
A measurement of the 238 U neutron-induced fission cross section was performed at the ORELA Linac facility in the neutron energy range between 5 eV and 3.5 MeV. The favorable signal-to-background ratio and high resolution of this experiment resulted in the identificaion of 85 subthreshold fission resonances or clusters of resonances in the neutron energy region between 5 eV and 200 keV. The fission data below 100 keV are characteristic of a weak coupling situation between Class I and Class II levels. The structure of the fission levels at the 720 eV and 1210 eV fission clusters is discussed. There is an apparent enhancement of the fission cross section at the opening of the 2 + neutron inelastic channel in 238 U at 45 keV. An enhancement of the subthreshold fission cross section between 100 keV and 200 keV is tentatively interpreted in terms of the presence of a Class II, partially damped vibrational level. There is a marked structure in the fission cross section above 200 keV up to and including the plateau between 2 and 3.5 MeV. 11 figures and 6 tables
Highlighted requests of neutron nuclear data measurements for fission reactors
International Nuclear Information System (INIS)
1977-01-01
Highlighted requests were selected from lists of requests for neutron nuclear Data measurements. This work was made by WRENDA Working Group of Japanese Nuclear Data Committee in response to an action of the NEANDC. This will be submitted to a NEA meeting on request lists. Compiled requests in this note correspond finally to the parts of the WRENDA 76/77 with some modifications and additional comments. (auth.)
Experimental study of fission process by fragment-neutron correlation measurement
Energy Technology Data Exchange (ETDEWEB)
Nishio, Katsuhisa; Yamamoto, Hideki; Kanno, Ikuo; Kimura, Itsuro; Nakagome, Yoshihiro [Kyoto Univ. (Japan). Faculty of Engineering
1997-07-01
Fragment-neutron correlation measurement of {sup 235}U(n{sub th}, f) was carried out. The obtained results showed more statistical accuracy than that of reported thermal neutron reaction. Experimental results and it`s analysis made clear the following facts. The minimum values of <{eta}> (m*) are shown at about 90 and 145 {mu} and <{eta}> (m*) showed the symmetrical form with an axis of symmetrical fission. This tendency is same as the distribution of {sup 252}Cf(s.f). -dV/dTKE(m*) indicates the saw-teethed distribution as same as <{nu}>(m*). The distribution seems depend on stiffness of fission fragment affected by the shell effect. The level density parameter a(m*) of fission fragment obtained from {sup 235}U(n{sub th}, f) expresses the saw-teethed distribution as same as that of {sup 252}Cf(s.f). This distribution can be explained by the empirical equation under consideration of the fission fragment depending on the shell effect and the collective motion. (S.Y.)
International Nuclear Information System (INIS)
Chiba, Go; Tsuji, Masashi; Narabayashi, Tadashi
2014-01-01
In order to properly quantify fission reactor neutronics parameter uncertainties, we have to use covariance data and sensitivity profiles consistently. In the present paper, we establish two consistent methodologies for uncertainty quantification: a self-shielded cross section-based consistent methodology and an infinitely-diluted cross section-based consistent methodology. With these methodologies and the covariance data of uranium-238 nuclear data given in JENDL-3.3, we quantify uncertainties of infinite neutron multiplication factors of light water reactor and fast reactor fuel cells. While an inconsistent methodology gives results which depend on the energy group structure of neutron flux and neutron-nuclide reaction cross section representation, both the consistent methodologies give fair results with no such dependences.
Delayed neutron spectra and their uncertainties in fission product summation calculations
Energy Technology Data Exchange (ETDEWEB)
Miyazono, T.; Sagisaka, M.; Ohta, H.; Oyamatsu, K.; Tamaki, M. [Nagoya Univ. (Japan)
1997-03-01
Uncertainties in delayed neutron summation calculations are evaluated with ENDF/B-VI for 50 fissioning systems. As the first step, uncertainty calculations are performed for the aggregate delayed neutron activity with the same approximate method as proposed previously for the decay heat uncertainty analyses. Typical uncertainty values are about 6-14% for {sup 238}U(F) and about 13-23% for {sup 243}Am(F) at cooling times 0.1-100 (s). These values are typically 2-3 times larger than those in decay heat at the same cooling times. For aggregate delayed neutron spectra, the uncertainties would be larger than those for the delayed neutron activity because much more information about the nuclear structure is still necessary. (author)
Directory of Open Access Journals (Sweden)
GO CHIBA
2014-06-01
Full Text Available In order to properly quantify fission reactor neutronics parameter uncertainties, we have to use covariance data and sensitivity profiles consistently. In the present paper, we establish two consistent methodologies for uncertainty quantification: a self-shielded cross section-based consistent methodology and an infinitely-diluted cross section-based consistent methodology. With these methodologies and the covariance data of uranium-238 nuclear data given in JENDL-3.3, we quantify uncertainties of infinite neutron multiplication factors of light water reactor and fast reactor fuel cells. While an inconsistent methodology gives results which depend on the energy group structure of neutron flux and neutron-nuclide reaction cross section representation, both the consistent methodologies give fair results with no such dependences.
Dosimetry of fission neutrons in a 1-W reactor, UTR-KINKI
Endo, S; Yoshitake, Y
2002-01-01
The energy spectrum of fission neutrons in the biological irradiation field of the Kinki University reactor, UTR-KINKI, has been determined by a multi-foil activation analysis coupled with artificial neural network techniques and a Au-foil activation method. The mean neutron energy was estimated to be 1.26+-0.05 MeV from the experimentally determined spectrum. Based on this energy value and other information, the neutron dose rate was estimated to be 19.7+-1.4 cGy/hr. Since this dose rate agrees with that measured by a pair of ionizing chambers (21.4 cGy/hr), we conclude that the mean neutron energy could be estimated with reasonable accuracy in the irradiation field of UTR-KINKI. (author)
Measurements of neutron-induced fission cross sections of Pb and Bi at intermediate energies
International Nuclear Information System (INIS)
Ryzhov, Igor; Tutin, Gennady; Eismont, Vilen; Mitryukhin, Andrey; Oplavin, Valery; Soloviev, Sergey; Conde, Henri; Olsson, Nils; Renberg, Per-Ulf
2002-01-01
Neutron-induced fission cross sections of nat Pb and 209 Bi have been measured relative to the 238 U(n.f) cross section at energies 96 MeV for lead and 133 MeV for bismuth. The measurements were performed at the quasi-mono-energetic neutron beam facility of The Svedberg Laboratory in Uppsala using Frisch-gridded ionization chamber. The results obtained are compared with other experimental data. The present state of the Bi standard recommended by IAEA is discussed. (author)
Thermal-neutron fission cross section of 26. 1-min /sup 235/U/sup m/
Energy Technology Data Exchange (ETDEWEB)
Talbert W.L. Jr.; Starner, J.W.; Estep, R.J.; Balestrini, S.J.; Attrep M. Jr.; Efurd, D.W.; Roensch, F.R.
1987-11-01
The thermal-neutron fission cross section of /sup 235/U/sup m/ has been measured relative to the ground-state cross section. A rapid radiochemical separation procedure was developed to provide sizeable (10/sup 10/ to 10/sup 11/ atom) samples that were reasonably free of the parent /sup 239/Pu. From a series of eight measurements, the value of 1.42 +- 0.04 was obtained for the ratio sigma/sub m//sigma/sub g/.
Japanese list of requests for neutron nuclear data for fission reactors
International Nuclear Information System (INIS)
Igarasi, Sin-iti; Asami, Tetsuo
1977-05-01
Requests for neutron nuclear data for fission reactors are presented. These are screened by a WRENDA Working Group of Japanese Nuclear Data Committee and submitted to WRENDA 76/77. This report includes 163 requests of which 55 requests are newly registered in the WRENDA. Three requests of the previous list are withdrawn. This activity is a part of the international cooperation with CCDN, NEANDC and INDC. (auth.)
Fast-neutron capture cross sections for the most important fission-product nuclei
International Nuclear Information System (INIS)
Gruppelaar, H.
1982-01-01
The main activity of the fission-product (FP) Working Group was the discussion of the current status of neutron capture knowledge of the most important FP nuclides, including the formulation of recommendations toward improved understanding. The results of the discussion are summarized. General conclusions and recommendations are given. The status of integral data is summarized by R. Anderl; and nuclear models and calculations are reviewed by D. Gardner and G. Reffo
International Nuclear Information System (INIS)
Constans, H.; Coville, P.; Guerre, J.
1975-01-01
Reactor control requires the determination of neutron flux at all times. The needed characteristics lead to use of several types of detectors: boron lined counters, boron lined ionization chambers, fission ionization chambers and self powered detectors. The principle of the reaction involved the fabrication requirements, the different modes of utilization and the characteristics obtained are examined for each detector. The problem of electric connections in the active area has been solved by developing ''integrated cables'' [fr
Spermatogenesis in adult rhesus monkeys following irradiation with X-rays or fission neutrons
International Nuclear Information System (INIS)
Rooij, D.G. de; Sonneveld, P.; Bekkum, D.W. van
A group of male rhesus monkeys was exposed to total body irradiation followed by autologous bone marrow transplantation. The animals were irradiated in the period between 1965 and 1976 and received a dose of 8.5 Gy of X-rays (300 KVP) or 3.6 Gy of 1 MeV fission neutrons. Of this group, a total of 11 male monkeys proved to be evaluable for studying the effects of irradiation on spermatogenesis. (Auth.)
Measurement of reaction cross sections of fission products induced by DT neutrons
Energy Technology Data Exchange (ETDEWEB)
Nakano, Daisuke; Murata, Isao; Takahashi, Akito [Osaka Univ., Suita (Japan)
1998-03-01
With the view of future application of fusion reactor to incineration of fission products, we have measured the {sup 129}I(n,2n){sup 128}I reaction cross section by DT neutrons with the activation method. The measured cross section was compared with the evaluated nuclear data of JENDL-3.2. From the result, it was confirmed that the evaluation overestimated the cross section by about 20-40%. (author)
International Nuclear Information System (INIS)
Alekseev, A.A.; Bergman, A.A.; Berlev, A.I.; Koptelov, E.A.; Egorov, A.S.; Samylin, B.F.; Trufanov, A.M.; Fursov, B.I.; Shorin, V.S.
2012-01-01
The neutron induced fission cross sections of Am and Cm isotopes were measured relative to 239 Pu in the neutron energy range from 1 eV to 20 keV at the INR RAS lead slowing down spectrometer LSDS-100. The fission resonance integrals were also estimated using the measured cross section data. The results have been compared with the available experimental and evaluated data. This analysis has shown the present status of the measured fission cross sections and the necessity to revise the evaluated cross sections libraries for the minor actinides. (author)
International Nuclear Information System (INIS)
Hirayama, Shoichi; Kawabe, Takaya
1995-01-01
The history of development of fusion power reactor has come to a turning point, where the main research target is now shifting from the plasma heating and confinement physics toward the burning plasma physics and reactor engineering. Although the development of fusion reactor system is the first time for human beings, engineers have experience of development of fission power reactor. The common feature between them is that both are plants used for the generation of nuclear reactions for the production of energy, nucleon, and radiation on an industrial scale. By studying the history of the development of the fission reactor, one can find the existence of experimental neutron reactors including irradiation facilities for fission reactor materials. These research neutron reactors played very important roles in the development of fission power reactors. When one considers the strategy of development of fusion power reactors from the points of fusion reactor engineering, one finds that the fusion neutron source corresponds to the neutron reactor in fission reactor development. In this paper, the authors discuss the roles of the plasma-based neutron source reactors in the development of fusion reactor engineering, by comparing it with the neutron reactors in the history of fission power development, and make proposals for the strategy of the fusion reactor development. 21 refs., 6 figs
International Nuclear Information System (INIS)
Isaev, S.G.; Piksaikin, L.E.; Kazakov, L.E.; Tarasko, M.Z.
2000-01-01
The measurements of relative abundances and periods of delayed neutrons from fast neutron induced fission of 235 U and 236 U have been made at the electrostatic accelerator CG-2.5 at IPPE. The preliminary results were obtained and discussed in the frame of the systematics of the average half-life of delayed neutron precursors. It was shown that the average half-life value in both reactions depends on the energy of primary neutrons [ru
International Nuclear Information System (INIS)
Unesaki, Hironobu; Shiroya, Seiji; Iwasaki, Tomohiko; Fujiwara, Daisuke; Kitada, Takanori; Kuroda, Mitsuo; Kohashi, Akio; Kato, Takeshi; Ikeuchi, Yoshitaka
2000-01-01
Integral measurements of 237 Np fission rate ratio relative to 235 U fission rate have been performed at Kyoto University Citrical Assembly. The fission rates have been measured using the back-to back type double fission chamber at five thermal cores with different H/ 235 U ratio so that the neutron spectra of the cores were systematically varied. The measured fission rate ratio per atom was 0.00439 to 0.0298, with a typical uncertainty of 2 to 3%. The measured data were compared with the calculated results using SRAC/TWOTRAN and MVP based on JENDL-3.2, which gave the averaged C/E values of 0.93 and 0.95, respectively. Obtained results of C/E using 237 Np cross sections from JENDL-3/2, ENDF/B-VI.5 and JEF2.2 show that the latter two gave smaller results than JENDL-3.2 by about 4%, which clearly reflects the discrepancy in the evaluated cross section among the libraries. This difference arises from both fast fission and resonance region. Although further improvement is recommended, 237 Np fission cross section in JENDL-3.2 is considered to be superior to those in the other libraries and can be adopted for use in design calculations for minor actinide transmutation system using thermal reactors with prediction precision of 237 Np fission rate with in 10%. (author)
Neutron-induced fission of uranium isotopes up to 100 MeV
International Nuclear Information System (INIS)
Lestone, J.P.; Gavron, A.
1994-01-01
The statistical-model description of the neutron-induced fission of U isotopes has been developed using densities of intrinsic states and spin cutoff parameters obtained directly from appropriate Nilsson model single-particle levels. The first-chance fission cross sections are reproduced well when the rotational contributions to the nuclear level densities are taken into account. In order to fit the U(n,f) cross sections above the threshold of second-chance fission, we must: (1) assume that the triaxial level-density enhancement is washed out at an excitation energy of approximately 7 MeV above the triaxial barriers with a width of approximately 1 MeV, implying a γ deformation for the first barriers where 10<γ<20 degree, and (2) include preequilibrium particle emission in the calculations. Above an incoming-neutron kinetic energy of approximately 17 MeV, our statistical model U(n,f) of cross sections increasingly overestimates the experimental data. This is not surprising since, at these high energies, little data exist on the scattering of neutrons to help guide the choice of optical-model parameters. A satisfactory reproduction of all of the available U(n,f) cross sections above 17 MeV is obtained by scaling our calculated compound-nucleus formation cross sections. This scaling factor falls from 1.0 at 17 MeV to 0.82 at 100 MeV
Energy Technology Data Exchange (ETDEWEB)
Badimon, C.; Barreau, G.; Doan, T.P.; Pedemay, G. [Centre d`Etudes Nucleaires, Bordeaux-1 Univ., 33 Gradignan (France); Gautherin, C.; Houry, M.; Korten, W.; Le Coz, Y.; Lucas, R.; Thiesen, Ch. [Dept. d`Astrophysique, de la Physique des Particules, de la Physique Nucleaire et de l`Instrumentation Associee, CEA Centre d`Etudes de Saclay, 91 - Gif-sur-Yvette (France); Belier, G.; Meot, M.V. [CEA Centre d`Etudes de Bruyeres-le-Chatel, 91 (France); Astier, A.; Ducroux, L.; Meyer, M.; Redon, N. [Inst.de Physique Nucleaire, Lyon-1 Univ., 69 - Villeurbanne (France)
1997-06-01
The prompt {gamma} emission in the spontaneous fission of {sup 252}Cf is characterized by an energy spectrum which extends up to 20 MeV. It was established that the spectrum presents in the neighbourhood of symmetric fission an intensity bump in the 3-8 MeV {gamma} energy interval. The origin of this phenomenon is still not well understood, so that it was found interesting to carry out new measurements. The spectrum of the {gamma} rays emitted in spontaneous fission of {sup 252}Cf has been measurement in the EUROGAM II multidetector using photovoltaic cells to detect fragments. The aim of the experiment was to investigate the {gamma} yield enhancement which appears for mass fragment ratio near 132/120. This enhancement was found to be composed of two peaks located at 4 MeV and 5.5 MeV respectively. The results obtained confirm the intensity bound in the 3-8 MeV region but this augmentation reaches the maximum when the heavy fragment is near the mass 132. Beyond mass 140 the phenomenon diminish and the {gamma} spectrum regains the behaviour expected for a statistic emission. The additional structure at 5.5 MeV does not vary with excitation energy while the excitation function of the 4 MeV structure is more structured and presents a maximum when the excitation energy is near 8 MeV. It is likely that all or part of this observed phenomenon is due to a particular excitation mode of this isotope associated for instance with a low energy dipole resonance. A theoretical study of this collective effect is under way 3 refs.
International Nuclear Information System (INIS)
Montoya, M.; Rojas, J.; Saetone, E.
2007-01-01
The mass and kinetic energy distribution of nuclear fragments from thermal neutron-induced fission of 235 U(n th ,f) have been studied using a Monte-Carlo simulation. Besides reproducing the pronounced broadening in the standard deviation of the kinetic energy at the final fragment mass number around m = 109, our simulation also produces a second broadening around m = 125. These results are in good agreement with the experimental data obtained by Belhafaf et al. and other results on yield of mass. We conclude that the obtained results are a consequence of the characteristics of the neutron emission, the sharp variation in the primary fragment kinetic energy and mass yield curves. We show that because neutron emission is hazardous to make any conclusion on primary quantities distribution of fragments from experimental results on final quantities distributions
International Nuclear Information System (INIS)
Bunatyan, G.G.; Nikolenko, V.G.; Popov, A.V.
2010-01-01
We treat the production of desirable radio isotopes due to the 238 U photo-fission by the bremsstrahlung induced in converter by an initial electron beam provided by a linear electron accelerator. We consider as well the radio isotope production through the 238 U fission by the neutrons that stem in the 238 U sample irradiated by that bremsstrahlung. The yield of the most applicable radio isotope 99 Mo is calculated. We correlate the findings acquired in the work presented with those obtained by treating the nuclear photo-neutron reaction. Menace of the plutonium contamination of an irradiated uranium sample because of the neutron capture by 238 U is considered. As we get convinced, the photo-neutron production of radio isotopes proves to be more practicable than the production by the uranium photo- and neutron-fission. Both methods are certain to be brought into action due to usage of the electron beam provided by modern linear accelerators
International Nuclear Information System (INIS)
Wagemans, C.
1979-01-01
Neutron induced and spontaneous fission with neutron energies from 10 -2 to 2.10 5 eV have been studied. Thermal neutron induced fission measurements in Pa 231 , Th 232 , Np 237 , U 233 , U 235 , Pu 239 and Pu 241 are reported. Energy and mass distributions of heavy fission fragments due to the spontaneous fission of Pu 240 are compared to the results obtained by thermal neutron fission of Pu 239 ; the events observed with U 236 , Pu 240 , Pa 232 and Np 238 are explained by the Bohr theory of fission channels. Ternary fission phenomena of U 233 , U 235 , Pu 239 , Pa 231 and Np 237 induced by thermal neutrons are explained and compared to models of Carjan and Feather. (MDC)
International Nuclear Information System (INIS)
Iunes, P.J.; Bigazzi, G.; Hadler Neto, J.C.; Laurenzi, M.A.; Balestrieri, M.L.; Norelli, P.; Osorio Araya, A.M.; Guedes, S.; Tello S, C.A.; Paulo, S.R.; Moreira, P.A.F.P.; Palissari, R.; Curvo, E.A.C.
2005-01-01
Neutron dosimetry based on U and Th thin films was used for fission-track dating of the age standard Moldavite, the central European tektite, from the Middle Miocene deposit of Jankov (southern Bohemia, Czech Republic). Our fission-track age (13.98+/-0.58Ma) agrees with a recent 40 Ar/ 39 Ar age, 14.34+/-0.04Ma, based on several determinations on Moldavites from different sediments, including the Jankov deposit. This result indicates that the U and Th thin film neutron dosimetry represents a reliable alternative for an absolute approach in fission-track dating
Energies and Yields of Prompt Gamma Rays from Fragments in Slow-Neutron Induced Fission of 235U
Energy Technology Data Exchange (ETDEWEB)
Albinsson, H [Chalmers Univ. of Technology, Goeteborg (SE)
1971-04-15
Measurements were made on the gamma radiation emitted from fission fragments in slow-neutron induced fission of 235U. The fragments were detected with solid state detectors of the surface barrier type and the gamma radiation with a Nal(Tl) scintillator. Mass selection was used so that the gamma radiation could be measured as a function of fragment mass. Time discrimination between the fission gammas and the prompt neutrons released in the fission process was employed to reduce the background. The gamma radiation emitted during different time intervals after the fission event was studied with the help of a collimator, the position of which was changed along the path of the fission fragments. In this way it was possible to select various collimator settings and let gamma radiation of different half-lives be enhanced. Gamma-ray energy spectra from these time components were then recorded as function of mass. The spectrum shape differed greatly depending on the half-life of the radiation and the fragment from which it was emitted. The results of the present measurements were discussed in the light of existing fission models, and comparisons were made with prompt gamma-ray and neutron data from other fission experiments
Energies and Yields of Prompt Gamma Rays from Fragments in Slow-Neutron Induced Fission of 235U
International Nuclear Information System (INIS)
Albinsson, H.
1971-04-01
Measurements were made on the gamma radiation emitted from fission fragments in slow-neutron induced fission of 235 U. The fragments were detected with solid state detectors of the surface barrier type and the gamma radiation with a Nal(Tl) scintillator. Mass selection was used so that the gamma radiation could be measured as a function of fragment mass. Time discrimination between the fission gammas and the prompt neutrons released in the fission process was employed to reduce the background. The gamma radiation emitted during different time intervals after the fission event was studied with the help of a collimator, the position of which was changed along the path of the fission fragments. In this way it was possible to select various collimator settings and let gamma radiation of different half-lives be enhanced. Gamma-ray energy spectra from these time components were then recorded as function of mass. The spectrum shape differed greatly depending on the half-life of the radiation and the fragment from which it was emitted. The results of the present measurements were discussed in the light of existing fission models, and comparisons were made with prompt gamma-ray and neutron data from other fission experiments
International Nuclear Information System (INIS)
Apperson, C.E. Jr.
1981-01-01
A method is presented for studying the influence of fission product transpot on delayed neutron precursors and decay heat sources during Liquid Metal Fast Breeder Reactor (LMFBR) unprotected accidents. The model represents the LMFBR core as a closed homogeneous cell. Thermodynamic phase equilibrium theory is used to predict fission product mobility. Reactor kinetics behavior is analyzed by an extension of point kinetics theory. Group dependent delayed neutron precursor and decay heat source retention factors, which represent the fraction of each group retained in the fuel, are developed to link the kinetics and thermodynamics analysis. Application of the method to a highly simplified model of an unprotected loss-of-flow accident shows a time delay on the order of 10 ms is introduced in the predisassembly power history if fission product motion is considered when compared to the traditional transient solution. The post-transient influence of fission product transport calculated by the present model is a 24 percent reduction in the decay heat level in the fuel material which is similar to traditional approximations. Isotopes of the noble gases, Kr and Xe, and the elements I and Br are shown to be very mobile and are responsible for a major part of the observed effects. Isotopes of the elements Cs, Se, Rb, and Te were found to be moderately mobile and contribute to a lesser extent to the observed phenomena. These results obtained from the application of the described model confirm the initial hypothesis that sufficient fission product transport can occur to influence a transient. For these reasons, it is concluded that extension of this model into a multi-cell transient analysis code is warranted
Energy Technology Data Exchange (ETDEWEB)
Moeller, Peter [Los Alamos National Laboratory, Theoretical Division, Los Alamos, NM (United States); Schmitt, Christelle [CEA/DSM-CNRS/IN2P3, Grand Accelerateur National d' Ions Lourds, Caen (France)
2017-01-15
We use the Brownian shape-motion model, with its recent extensions, which allow modeling of odd-even staggering, to calculate the evolution of fission-fragment charge distributions with neutron number for the compound-system sequence {sup 234}U, {sup 236}U, {sup 238}U, and {sup 240}U. We compare to experimental data where available, for neutron- and electromagnetic-induced fission over a compound-nucleus excitation energy range from about 6 to 20 MeV. A notable result of the study is that the evolution of the location of the peak charge yield from Z = 54 in {sup 234}U towards Z = 52 in heavier isotopes, seen in the experimental data, is present also in the calculated yields. We further show that to describe yields at higher compound-nucleus excitation energies, then, already at 20 MeV, it is necessary to take multi-chance fission into account. (orig.)
Features of the neutron spectra accompanying the fission of actinide nuclei
International Nuclear Information System (INIS)
Lovchikova, G.N.; Trufanov, A.M.; Svirin, M.I.; Polyakov, A.V.; Vinogradov, V.A.; Dmitriev, V.D.; Boykov, G.S.
2000-01-01
The spectra of fission neutrons from 238 U are measured by the time-of-flight technique at incident-neutron energies E n = 5.0 and 13.2 MeV. The data are compared with those obtained in the previous studies for 232 Th, 235,238 U, 237 Np at E n = 2.9 and 14.7 MeV; for 232 Th at E n = 14.6 and 17.7 MeV; for 238 U at 16.0 and 17.7 MeV. An excess of soft neutrons, which is observed in comparing experimental spectra for E n 13.2, 14.7, 16.0 and 17.7 MeV with the results of traditional theoretical calculations, is reproduced fairly well under the assumption that, at high excitation energies of a compound system, some part of post-fission neutrons can be emitted by nonaccelerated fragments [ru
Spectral effects in low-dose fission and fusion neutron irradiated metals and alloys
International Nuclear Information System (INIS)
Heinisch, H.L.; Atkin, S.D.; Martinez, C.
1986-04-01
Flat miniature tensile specimens were irradiated to neutron fluences up to 9 x 10 22 n/m 2 in the RTNS-II and in the Omega West Reactor. Specimen temperatures were the same in both environments, with runs being made at both 90 0 C and 290 0 C. The results of tensile tests on AISI 316 stainless steel, A302B pressure vessel steel and pure copper are reported here. The radiation-induced changes in yield strength as a function of neutron dose in each spectrum are compared. The data for 316 stainless steel correlate well on the basis of displacements per atom (dpa), while those for copper and A302B do not. In copper the ratio of fission dpa to 14 MeV neutron dpa for a given yield stress change is about three to one. In A302B pressure vessel steel this ratio is more than three at lower fluences, but the yield stress data for fission and 14 MeV neutron-irradiated A302B steel appears to coalesce or intersect at the higher fluences
Energy Technology Data Exchange (ETDEWEB)
O' Rourke, Patrick Francis [Los Alamos National Lab. (LANL), Los Alamos, NM (United States)
2016-10-27
The purpose of this report is to provide the reader with an understanding of how a Monte Carlo neutron transport code was written, developed, and evolved to calculate the probability distribution functions (PDFs) and their moments for the neutron number at a final time as well as the cumulative fission number, along with introducing several basic Monte Carlo concepts.
Measurement of the fission cross-section ratio for 237Np/235U around 14 MeV neutron energies
International Nuclear Information System (INIS)
Desdin, L.; Szegedy, S.; Csikai, J.
1989-01-01
Fission cross-section ratio was determined for 237 Np/ 235 U around 14 MeV neutron energies with a back-to-back ionization chamber. Neutrons were produced by a 180 KV accelerator using T(d,n) 4 He reaction. No significant energy dependence was found in the cross section ratio
Application of modular neutron spectrometer to measure neutron spectra from fission of 252Cf
International Nuclear Information System (INIS)
Szeflinski, Z.; Osuch, S.; Popkiewicz, M.; Wilhelmi, Z.; Zelazny, Z.
1996-01-01
The neutron spectrometer MONA (Modular Neutron Array) and its test has been described. The spectrometers consist of eight BC-501A liquid scintillator detectors of BICRON which allow one to distinguish between the pulses from gamma quanta and neutrons using pulse shape discrimination (PSD) method. The electronic equipment for the PSD and the test result using the 252 Cf radioactive source are presented
International Nuclear Information System (INIS)
Martin, Julie-Fiona; Taieb, Julien; Chatillon, Audrey; Belier, Gilbert; Boutoux, Guillaume; Ebran, Adeline; Gorbinet, Thomas; Grente, Lucie; Laurent, Benoit; Pellereau, Eric; Alvarez-Pol, Hector; Ayyad, Yassid; Benlliure, Jose; Cortina Gil, Dolores; Caamano, Manuel; Fernandez Dominguez, Beatriz; Paradela, Carlos; Ramos, Diego; Rodriguez-Sanchez, Jose-Luis; Vargas, Jossitt; Audouin, Laurent; Tassan-Got, Laurent; Aumann, Thomas; Casarejos, Enrique; Farget, Fanny; Rodriguez-Tajes, Carme; Heinz, Andreas; Jurado, Beatriz; Kelic-Heil, Aleksandra; Kurz, Nikolaus; Nociforo, Chiara; Pietri, Stephane; Rossi, Dominic; Schmidt, Karl-Heinz; Simon, Haik; Voss, Bernd; Weick, Helmut
2015-01-01
A novel technique for fission studies, based on the inverse kinematics approach, is presented. Following pioneering work in the nineties, the SOFIA Collaboration has designed and built an experimental set-up dedicated to the simultaneous measurement of isotopic yields, total kinetic energies and total prompt neutron multiplicities, by fully identifying both fission fragments in coincidence, for the very first time. This experiment, performed at GSI, permits to study the fission of a wide variety of fissioning systems, ranging from mercury to neptunium, possibly far from the valley of stability. A first experiment, performed in 2012, has provided a large array of unprecedented data regarding the nuclear fission process. An excerpt of the results is presented. With this solid starter, further improvements of the experimental set-up are considered, which are consistent with the expected developments at the GSI facility, in order to measure more fission observables in coincidence. The completeness reached in the SOFIA data, permits to scrutinize the correlations between the interesting features of fission, offering a very detailed insight in this still unraveled mechanism. (orig.)
Energy Technology Data Exchange (ETDEWEB)
Martin, Julie-Fiona; Taieb, Julien; Chatillon, Audrey; Belier, Gilbert; Boutoux, Guillaume; Ebran, Adeline; Gorbinet, Thomas; Grente, Lucie; Laurent, Benoit; Pellereau, Eric [CEA DAM Bruyeres-le-Chatel, Arpajon (France); Alvarez-Pol, Hector; Ayyad, Yassid; Benlliure, Jose; Cortina Gil, Dolores; Caamano, Manuel; Fernandez Dominguez, Beatriz; Paradela, Carlos; Ramos, Diego; Rodriguez-Sanchez, Jose-Luis; Vargas, Jossitt [Universidad de Santiago de Compostela, Santiago de Compostela (Spain); Audouin, Laurent; Tassan-Got, Laurent [CNRS/IN2P3, IPNO, Orsay (France); Aumann, Thomas [Technische Universitaet Darmstadt, Darmstadt (Germany); Casarejos, Enrique [Universidad de Vigo, Vigo (Spain); Farget, Fanny; Rodriguez-Tajes, Carme [CNRS/IN2P3, GANIL, Caen (France); Heinz, Andreas [Chalmers University of Technology, Gothenburg (Sweden); Jurado, Beatriz [CNRS/IN2P3, CENBG, Gradignan (France); Kelic-Heil, Aleksandra; Kurz, Nikolaus; Nociforo, Chiara; Pietri, Stephane; Rossi, Dominic; Schmidt, Karl-Heinz; Simon, Haik; Voss, Bernd; Weick, Helmut [GSI Helmholtzzentrum fuer Schwerionenforschung GmbH, Darmstadt (Germany)
2015-12-15
A novel technique for fission studies, based on the inverse kinematics approach, is presented. Following pioneering work in the nineties, the SOFIA Collaboration has designed and built an experimental set-up dedicated to the simultaneous measurement of isotopic yields, total kinetic energies and total prompt neutron multiplicities, by fully identifying both fission fragments in coincidence, for the very first time. This experiment, performed at GSI, permits to study the fission of a wide variety of fissioning systems, ranging from mercury to neptunium, possibly far from the valley of stability. A first experiment, performed in 2012, has provided a large array of unprecedented data regarding the nuclear fission process. An excerpt of the results is presented. With this solid starter, further improvements of the experimental set-up are considered, which are consistent with the expected developments at the GSI facility, in order to measure more fission observables in coincidence. The completeness reached in the SOFIA data, permits to scrutinize the correlations between the interesting features of fission, offering a very detailed insight in this still unraveled mechanism. (orig.)
Energy Technology Data Exchange (ETDEWEB)
Glumac, B [Institut Jozef Stefan, Ljubljana (Yugoslavia)
1979-07-01
After the reconstruction of the exposure room of the TRIGA reactor a new measurement of the neutron spectrum behind the fission converter was necessary. The multiple foil method was applied. Following twelve reactions were chosen: 197-Au (n, {gamma}), 63-Cu (n, {gamma}), 59-Co (n, {gamma}), 115-In (n.n'), 64-Zn )n.p), 27-Al (n, {alpha}), 25 Mg (n,p), 56-Fe (n,p), 19 F (n,2n'), 237-Np (n,f), 239 Pu (n,f) and 235-U (n,f). The neutron spectrum was calculated from measured reaction rates using our unfolding code ITERAD. The neutron cross sections library DOCROS 77 was applied for the calculations. (author)
Formation and distribution of fragments in the spontaneous fission of 240Pu
Sadhukhan, Jhilam; Zhang, Chunli; Nazarewicz, Witold; Schunck, Nicolas
2017-12-01
Background: Fission is a fundamental decay mode of heavy atomic nuclei. The prevalent theoretical approach is based on mean-field theory and its extensions where fission is modeled as a large amplitude motion of a nucleus in a multidimensional collective space. One of the important observables characterizing fission is the charge and mass distribution of fission fragments. Purpose: The goal of this Rapid Communication is to better understand the structure of fission fragment distributions by investigating the competition between the static structure of the collective manifold and the stochastic dynamics. In particular, we study the characteristics of the tails of yield distributions, which correspond to very asymmetric fission into a very heavy and a very light fragment. Methods: We use the stochastic Langevin framework to simulate the nuclear evolution after the system tunnels through the multidimensional potential barrier. For a representative sample of different initial configurations along the outer turning-point line, we define effective fission paths by computing a large number of Langevin trajectories. We extract the relative contribution of each such path to the fragment distribution. We then use nucleon localization functions along effective fission pathways to analyze the characteristics of prefragments at prescission configurations. Results: We find that non-Newtonian Langevin trajectories, strongly impacted by the random force, produce the tails of the fission fragment distribution of 240Pu. The prefragments deduced from nucleon localizations are formed early and change little as the nucleus evolves towards scission. On the other hand, the system contains many nucleons that are not localized in the prefragments even near the scission point. Such nucleons are distributed rapidly at scission to form the final fragments. Fission prefragments extracted from direct integration of the density and from the localization functions typically differ by more than
International Nuclear Information System (INIS)
Wang Dahai.
1990-10-01
The main objectives of this IAEA Co-ordinated Research Programme are to improve the data on 14 MeV neutron-induced double-differential neutron emission cross sections for materials needed for fission and fusion reactor technology. This report summarizes the conclusions and recommendations which were agreed by all participants during the Second Research Co-ordination Meeting
International Nuclear Information System (INIS)
Pál, L.; Pázsit, I.
2015-01-01
The signals of fission chambers are usually evaluated with the help of the co-called Campbelling techniques. These are based on the Campbell theorem, which states that if the primary incoming events, generating the detector pulses, are independent, then relationships exist between the moments of various orders of the signal in the current mode. This gives the possibility to determine the mean value of the intensity of the detection events, which is proportional to the static flux, from the higher moments of the detector current, which has certain advantages. However, the main application area of fission chambers is measurements in power reactors where, as is well known, the individual detection events are not independent, due to the branching character of the neutron chains (neutron multiplication). Therefore it is of interest to extend the Campbelling-type theory for the case of correlated neutron events. Such a theory could address two questions: partly, to investigate the bias when the traditional Campbell techniques are used for correlated incoming events; and partly, to see whether the correlation properties of the detection events, which carry information on the multiplying medium, could be extracted from the measurements. This paper is devoted to the investigation of these questions. The results show that there is a potential possibility to extract the same information from fission chamber signals in the current mode as with the Rossi- or Feynman-alpha methods, or from coincidence and multiplicity measurements, which so far have required detectors working in the pulse mode. It is also shown that application of the standard Campbelling techniques to neutron detection in multiplying systems does not lead to an error for estimating the stationary flux as long as the detector is calibrated in in situ measurements
Optimizing moderation of He-3 neutron detectors for shielded fission sources
Energy Technology Data Exchange (ETDEWEB)
Rees, Lawrence B., E-mail: Lawrence_Rees@byu.edu [Department of Physics and Astronomy, Brigham Young University, Provo, UT 84602 (United States); Czirr, J. Bart, E-mail: czirr@juno.com [Department of Physics and Astronomy, Brigham Young University, Provo, UT 84602 (United States)
2012-11-01
The response of a {sup 3}He neutron detector is highly dependent on the amount of moderator incorporated into the detector system. If there is too little moderation, neutrons will not react with the {sup 3}He. If there is too much moderation, neutrons will not reach the {sup 3}He. In applications for portal or border monitors where {sup 3}He detectors are used to interdict illicit importation of plutonium, the fission source is always shielded to some extent. Since the energy distribution of neutrons emitted from the source depends on the amount and type of shielding present, the optimum placement of moderating material around {sup 3}He tubes is a function of shielding. In this paper, we use Monte Carlo techniques to model the response of {sup 3}He tubes placed in polyethylene boxes for moderation. To model the shielded fission neutron source, we use a point {sup 252}Cf source placed in the center of polyethylene spheres of varying radius. Detector efficiency as a function of box geometry and shielding is explored. We find that increasing the amount of moderator behind and to the sides of the detector generally improves the detector response, but that incremental benefits are minimal if the thickness of the polyethylene moderator is greater than about 5-7 cm. The thickness of the moderator in front of the {sup 3}He tubes, however, is very important. For bare sources, about 4-5 cm of moderator is optimum, but as the shielding increases, the optimum thickness of this moderator decreases to 0.5-1 cm. Similar conclusions can be applied to polyethylene boxes employing two {sup 3}He tubes. Two-tube boxes with front moderators of non-uniform thickness may be useful for detecting neutrons over a wide energy range.
Progress in fission product nuclear data. No. 13
International Nuclear Information System (INIS)
Lammer, M.
1990-11-01
This is the 13th issue of a report series published by the Nuclear Data Section of the IAEA. The types of activities included are measurements, compilations and evaluations of: Fission product yields (neutron induced and spontaneous fission), neutron reaction cross-sections of fission products, data related to the radioactive decay of fission products, delayed neutron data of fission products and bumped fission product data (decay heat, absorption, etc.). The first part of the report consists of unaltered original data which the authors have sent to IAEA/NDS. The second part contains some recent references relative to fission product nuclear data, which were not covered by the contributions submitted, and selected papers from conferences. Part 3 contains requirements for further measurements
Progress in fission product nuclear data. No. 14
International Nuclear Information System (INIS)
Lammer, M.
1994-06-01
This is the 14th issue of a report series on Fission Product Nuclear Data published by the Nuclear Data Section of the IAEA. The types of activities included are measurements, compilations and evaluations of fission product yields, neutron reaction cross sections of fission products, data related to the radioactive decay of fission products, delayed neutron data from neutron induced and spontaneous fission, lumped fission product data. The first part of the report consists of unaltered original contributions which the authors have sent to IAEA/NDS. The second part contains some recent references relative to fission product nuclear data, which were not covered by the contributions submitted, and selected papers from conferences. The third part contains requirements for further measurements
International Nuclear Information System (INIS)
Dulugeac, S. D.; Mladin, M.; Budriman, A. G.
2013-01-01
Molybdenum production can be a solution for the future in the utilization of the Romanian TRIGA, taking into account the international market supply needs. Generally, two different techniques are available for Mo 99 production for use in medical Tc 99 generation.The first one is based on neutron irradiation of molybdenum targets of natural isotopic composition or enriched in Mo 98 . In a second process, Mo 99 is obtained as a result of the neutron induced fission of U 235 according to U 235 (n,f) Mo 99 . The objectives of the paper are related to Mo 99 production as a result of fission. Neutron physics parameters are determined and presented, such as: thermal flux axial distribution for the critical reactor at 10 MW inside the irradiation location; reactivity introduced by three Uranium foil containers; neutron fluxes and fission rates in the Uranium foils; released and deposited power in the Uranium foils; Mo 99 activity in the Uranium foils. (authors)
Energy partition in nuclear fission
International Nuclear Information System (INIS)
Ruben, A.; Maerten, H.; Seeliger, D.
1990-01-01
A scission point model (two spheroid model TSM) including semi-empirical temperature-dependent shell correction energies for deformed fragments at scission is presented. It has been used to describe the mass-asymmetry-dependent partition of the total energy release on both fragments from spontaneous and induced fission. Characteristic trends of experimental fragment energy and neutron multiplicity data as function of incidence energy in the Th-Cf region of fissioning nuclei are well reproduced. Based on model applications, information on the energy dissipated during the descent from second saddle of fission barrier to scission point have been deduced. (author). 39 refs, 13 figs
Exploratory analysis of a neutron-rich nuclei source based on photo-fission
Mirea, M; Clapier, F; Essabaa, S; Groza, L; Ibrahim, F; Kandri-Rody, S; Müller, A C; Pauwels, N; Proust, J
2003-01-01
A source of neutron rich ions can be conceived through the photo-fission process. An exploratory study of such a source is realized. A survey of the radiative electron energy loss theory is reported in order to estimate numerically the bremsstrahlung production of thick targets. The resulted bremsstrahlung angular and energy theoretical distributions delivered from W and UCx thick converters are presented and compared with previous results. Some quantities as the number of fission events produced in the fissionable source and the energy loss in the converters are also reported as function of the geometry of the combination and the incident electron energy. An attempt of comparison with experimental data shows a quantitative agreement. This study is focussed on initial kinetic energies of the electron beam included in the range 30-60 MeV, suitable for the production of large radiative gamma-ray yields able to induce the $^{238}$U fission through the giant dipole resonance. A confrontation with the number of fi...
Fission barrier theory and its application to the calculation of actinide neutron cross-sections
International Nuclear Information System (INIS)
Lynn, J.E.
1980-01-01
The lectures discuss the possibilities and realisations of applying nuclear fission theory to the calculation of unknown nuclear data required for applications, principally in the nuclear power field. A brief description of the fundamentals of fission theory, the nature of the potential energy surface in the deformation plane, and of the inertial tensor, is given, and the accuracy of the theoretical calculations is discussed. It is concluded that it is impracticable to obtain required quantities such as neutron cross-sections from such fundamental calculations at present. On the other hand the fundamental theory reveals a wealth of phenomenological aspects of the fission process which can be incorporated into nuclear reaction theory. It is then shown how reaction theory thus extended to take correct account of the structured (''double-humped'') fission barrier can be used to parametrise the barrier by analysis of experimental data, and subsequently to calculate new data. Descriptions of computer programmes and illustrations of the application of the methods to actual physical examples are included in this account. (author)
Calculation of neutron importance function in fissionable assemblies using Monte Carlo method
International Nuclear Information System (INIS)
Feghhi, S.A.H.; Shahriari, M.; Afarideh, H.
2007-01-01
The purpose of the present work is to develop an efficient solution method for the calculation of neutron importance function in fissionable assemblies for all criticality conditions, based on Monte Carlo calculations. The neutron importance function has an important role in perturbation theory and reactor dynamic calculations. Usually this function can be determined by calculating the adjoint flux while solving the adjoint weighted transport equation based on deterministic methods. However, in complex geometries these calculations are very complicated. In this article, considering the capabilities of MCNP code in solving problems with complex geometries and its closeness to physical concepts, a comprehensive method based on the physical concept of neutron importance has been introduced for calculating the neutron importance function in sub-critical, critical and super-critical conditions. For this propose a computer program has been developed. The results of the method have been benchmarked with ANISN code calculations in 1 and 2 group modes for simple geometries. The correctness of these results has been confirmed for all three criticality conditions. Finally, the efficiency of the method for complex geometries has been shown by the calculation of neutron importance in Miniature Neutron Source Reactor (MNSR) research reactor
Multiplicity and energy of neutrons from {sup 233}U(n{sub th},f) fission fragments
Energy Technology Data Exchange (ETDEWEB)
Nishio, Katsuhisa; Kimura, Itsuro; Nakagome, Yoshihiro [Kyoto Univ. (Japan)
1998-03-01
The correlation between fission fragments and prompt neutrons from the reaction {sup 233}U(n{sub th},f) was measured with improved accuracy. The results determined the neutron multiplicity and emission energy as a function of fragment mass and total kinetic energy. The average energy as a function of fragment mass followed a nearly symmetric distribution centered about the equal mass-split and formed a remarkable contrast with the saw-tooth distribution of the average neutron multiplicity. The neutron multiplicity from the specified fragment decreases linearly with total kinetic energy, and the slope of multiplicity with kinetic energy had the minimum value at about 130 u. The level density parameter versus mass determined from the neutron data showed a saw-tooth structure with the pronounced minimum at about 128 and generally followed the formula by Gilbert and Cameron, suggesting that the neutron emission process was very much affected by the shell-effect of the fission fragment. (author)
Energy Technology Data Exchange (ETDEWEB)
Kramer, Kevin James [Univ. of California, Berkeley, CA (United States)
2010-04-08
This study investigates the neutronics design aspects of a hybrid fusion-fission energy system called the Laser Fusion-Fission Hybrid (LFFH). A LFFH combines current Laser Inertial Confinement fusion technology with that of advanced fission reactor technology to produce a system that eliminates many of the negative aspects of pure fusion or pure fission systems. When examining the LFFH energy mission, a significant portion of the United States and world energy production could be supplied by LFFH plants. The LFFH engine described utilizes a central fusion chamber surrounded by multiple layers of multiplying and moderating media. These layers, or blankets, include coolant plenums, a beryllium (Be) multiplier layer, a fertile fission blanket and a graphite-pebble reflector. Each layer is separated by perforated oxide dispersion strengthened (ODS) ferritic steel walls. The central fusion chamber is surrounded by an ODS ferritic steel first wall. The first wall is coated with 250-500 μm of tungsten to mitigate x-ray damage. The first wall is cooled by Li_{17}Pb_{83 } eutectic, chosen for its neutron multiplication and good heat transfer properties. The Li_{17}Pb_{83} flows in a jacket around the first wall to an extraction plenum. The main coolant injection plenum is immediately behind the Li_{17}Pb_{83}, separated from the Li_{17}Pb_{83} by a solid ODS wall. This main system coolant is the molten salt flibe (2LiF-BeF_{2}), chosen for beneficial neutronics and heat transfer properties. The use of flibe enables both fusion fuel production (tritium) and neutron moderation and multiplication for the fission blanket. A Be pebble (1 cm diameter) multiplier layer surrounds the coolant injection plenum and the coolant flows radially through perforated walls across the bed. Outside the Be layer, a fission fuel layer comprised of depleted uranium contained in Tristructural-isotropic (TRISO) fuel particles
Energy Technology Data Exchange (ETDEWEB)
Caizergues, R; Clouet d' Orval, C [Commissariat a l' Energie Atomique, Saclay (France).Centre d' Etudes Nucleaires
1960-07-01
It is very important to know the plutonium-240 content of the plutonium formed in piles. The method of measurement described here consists in counting the number of spontaneous fissions produced in a known quantity of plutonium. This measurement is carried out in a multiple-plate ionisation chamber, the plutonium being deposited on the plates. The disintegration constant of plutonium-240 by spontaneous fission being known the plutonium-240 content in the sample can be calculated. (author) [French] La connaissance de la teneur en plutonium-240 du plutonium forme dans les piles est une question importante. La methode de mesure presentee ici consiste a compter le nombre de fissions spontanees issues d'une quantite connue de plutonium. Cette mesure est effectuee dans une chambre d'ionisation a plateaux multiples sur lesquels est depose le plutonium. La connaissance de la constante de desintegration du plutonium-240 par fissions spontanees permet de calculer la teneur en plutonium-240. (auteur)
Fission neutron spectrum averaged cross sections for threshold reactions on arsenic
International Nuclear Information System (INIS)
Dorval, E.L.; Arribere, M.A.; Kestelman, A.J.; Comision Nacional de Energia Atomica, Cuyo Nacional Univ., Bariloche; Ribeiro Guevara, S.; Cohen, I.M.; Ohaco, R.A.; Segovia, M.S.; Yunes, A.N.; Arrondo, M.; Comision Nacional de Energia Atomica, Buenos Aires
2006-01-01
We have measured the cross sections, averaged over a 235 U fission neutron spectrum, for the two high threshold reactions: 75 As(n,p) 75 mGe and 75 As(n,2n) 74 As. The measured averaged cross sections are 0.292±0.022 mb, referred to the 3.95±0.20 mb standard for the 27 Al(n,p) 27 Mg averaged cross section, and 0.371±0.032 mb referred to the 111±3 mb standard for the 58 Ni(n,p) 58m+g Co averaged cross section, respectively. The measured averaged cross sections were also evaluated semi-empirically by numerically integrating experimental differential cross section data extracted for both reactions from the current literature. The calculations were performed for four different representations of the thermal-neutron-induced 235 U fission neutron spectrum. The calculated cross sections, though depending on analytical representation of the flux, agree with the measured values within the estimated uncertainties. (author)
Determination of technetium-99 in mixed fission products by neutron activation analysis
International Nuclear Information System (INIS)
Bate, L.C.
1980-01-01
A method has been developed for analysis of 99 Tc in fission product mixtures. The analysis consists of a chemical separation of 99 Tc, neutron irradiation of the isolated 99 Tc, and gamma-ray spectrometric determination of the induced 100 Tc radioactivity. Technetium-99 is chemically separated from most fission products by a cyclohexanone extraction from basic carbonate solution. Technetium-99 is stripped into water by addition of carbon tetrachloride to the cyclohexanone phase. A final step in the separation procedure is adsorption of 99 Tc on an anion exchange column which provides additional decontamination and places the 99 Tc in a concentrated form for neutron activation analysis. Neutron irradiations of the isolated 99 Tc were made in the pneumatic tube facility at the High Flux Isotope Reactor at a flux of 5 x 10 14 n/cm 2 /sec for 11 seconds. Induced 100 Tc radioactivity was determined immediately after irradiation using gamma-ray spectrometry to measure the 540 and 591 keV lines. Sensitivity of the analysis under these conditions is approximately 5 ng, and samples of up to about 100 ml volume can be easily processed. The method has been successfully applied to reactor fuel solutions and off-gas traps containing 6.5 x 10 -4 to 240 μg 99 Tc/ml
International Nuclear Information System (INIS)
Sirinuntavid, Alice; Rodthongkom, Chouvana
2007-08-01
Full text: Comparison between Neutron Activation Analysis (NAA) and fission track technique for uranium determination in solid samples was studied by use of standard reference materials, i.e., ore, coal fly ash, soil. For NAA, the epithermal neutron was applied for activated irradiation. Then, the 74.5 keV gamma from U-239 or 277.7 keV gamma from Np-239 was measured. For high Uranium content samples, NAA method with 74.5 keV gamma measurement, gave higher precision result than the 277.7 keV gamma measurement method. NAA method with 277.7 keV gamma measurement, gave higher sensitivity and precision result for low Uranium content samples and the uranium contained less than 10 ppm samples. Nevertheless, the latter procedure needed longer time for neutron irradiation and analysis procedure. In comparison the results of Uranium analysis between NAA and fission track, it was found that no significant difference within 95 % of confidence level
Energy Technology Data Exchange (ETDEWEB)
Morrison, Samuel S.; Clark, Sue B.; Eggemeyer, Tere A.; Finn, Erin C.; Hines, C. Corey; King, Mathew D.; Metz, Lori A.; Morley, Shannon M.; Snow, Mathew S.; Wall, Donald E.; Seiner, Brienne N.
2017-11-02
Activation analysis of gold (Au) is used to estimate neutron fluence resulting from a criticality event; however, such analyses are complicated by simultaneous production of other gamma-emitting fission products. Confidence in neutron fluence estimates can be increased by quantifying additional activation products such as platinum (Pt), tantalum (Ta), and tungsten (W). This work describes a radiochemical separation procedure for the determination of these activation products. Anion exchange chromatography is used to separate anionic forms of these metals in a nitric acid matrix; thiourea is used to isolate the Au and Pt fraction, followed by removal of the Ta fraction using hydrogen peroxide. W, which is not retained on the first anion exchange column, is transposed to an HCl/HF matrix to enhance retention on a second anion exchange column and finally eluted using HNO3/HF. Chemical separations result in a reduction in the minimum detectable activity by a factor of 287, 207, 141, and 471 for 182Ta, 187W, 197Pt, and 198Au respectively, with greater than 90% recovery for all elements. These results represent the highest recoveries and lowest minimum detectable activities for 182Ta, 187W, 197Pt, and 198Au from mixed fission-activation product samples to date, enabling considerable refinement in the measurement uncertainties for neutron fluences in highly complex sample matrices.
Shi, Xue-Ming; Peng, Xian-Jue
2016-09-01
Fusion science and technology has made progress in the last decades. However, commercialization of fusion reactors still faces challenges relating to higher fusion energy gain, irradiation-resistant material, and tritium self-sufficiency. Fusion Fission Hybrid Reactors (FFHR) can be introduced to accelerate the early application of fusion energy. Traditionally, FFHRs have been classified as either breeders or transmuters. Both need partition of plutonium from spent fuel, which will pose nuclear proliferation risks. A conceptual design of a Fusion Fission Hybrid Reactor for Energy (FFHR-E), which can make full use of natural uranium with lower nuclear proliferation risk, is presented. The fusion core parameters are similar to those of the International Thermonuclear Experimental Reactor. An alloy of natural uranium and zirconium is adopted in the fission blanket, which is cooled by light water. In order to model blanket burnup problems, a linkage code MCORGS, which couples MCNP4B and ORIGEN-S, is developed and validated through several typical benchmarks. The average blanket energy Multiplication and Tritium Breeding Ratio can be maintained at 10 and 1.15 respectively over tens of years of continuous irradiation. If simple reprocessing without separation of plutonium from uranium is adopted every few years, FFHR-E can achieve better neutronic performance. MCORGS has also been used to analyze the ultra-deep burnup model of Laser Inertial Confinement Fusion Fission Energy (LIFE) from LLNL, and a new blanket design that uses Pb instead of Be as the neutron multiplier is proposed. In addition, MCORGS has been used to simulate the fluid transmuter model of the In-Zinerater from Sandia. A brief comparison of LIFE, In-Zinerater, and FFHR-E will be given.
Energy Technology Data Exchange (ETDEWEB)
Kerr, P. L. [Lawrence Livermore National Lab. (LLNL), Livermore, CA (United States)
2017-02-28
An SNM attribute Information Barrier (IB) system was developed for a 2011 US/UK Exercise. The system was modified and extensively tested in a 2013-2014 US-UK Measurement Campaign. This work demonstrated rapid deployment of an IB system for potential treaty use. The system utilizes an Ortec Fission Meter neutron multiplicity counter and custom computer code. The system demonstrates a proof-of-principle automated Pu-240 mass determination with an information barrier. After a software start command is issued, the system automatically acquires and downloads data, performs an analysis, and displays the results. This system conveys the results of a Pu mass threshold measurements in a way the does not reveal sensitive information. In full IB mode, only red/green ‘lights’ are displayed in the software. In test mode, more detailed information is displayed. The code can also read in, analyze, and display results from previously acquired or simulated data. Because the equipment is commercial-off-the-shelf (COTS), the system demonstrates a low-cost short-lead-time technology for treaty SNM attribute measurements. A deployed system will likely require integration of additional authentication and tamper-indicating technologies. This will be discussed for the project in this and future progress reports.
Radiochemical studies on fission
Energy Technology Data Exchange (ETDEWEB)
None
1973-07-01
Research progress is reported on nuclear chemistry; topics considered include: recoil range and kinetic energy distribution in the thermal neutron ftssion of /sup 245/Cm; mass distribution and recoil range measurements in the reactor neutron-induced fission of /sup 232/U; fission yields in the thermal neutron fission of /sup 241/PU highly asymmetric binary fission of uranium induced by reactor neutrons; and nuclear charge distribution in low energy fission. ( DHM)
Thermal-Neutron-Induced Fission of U235, U233 and Pu239
International Nuclear Information System (INIS)
Thomas, T.D.; Gibson, W.M.; Safford, G.J.
1965-01-01
We have used solid-state detectors to measure the kinetic energies of the coincident fission fragments in the thermal-neutron-induced fission of U 235 , U 233 and Pu 239 . Special care has been taken to eliminate spurious-events near symmetry to give an accurate measure of such quantities as the average total kinetic energy at symmetry. For each fissioning system over 10 6 events were recorded. As a result the statistics are good enough to see definite evidence for fine structure over a wide range of masses and energies. The data have been analysed to give mass yield curves, average kinetic energies as a function of mass, and other quantities of interest. For each fissioning system the average total kinetic energy goes through a maximum for a heavy fragment mass of about 132 and for the corresponding light fragment mass. There is a pronounced minimum at symmetry, although not as deep as that found in time-of-flight experiments. The difference between the maximum average kinetic energy and that at symmetry is about 32 MeV for U 235 , 18 MeV for U 233 and 20 MeV for Pu 239 . The dispersion of kinetic energies at symmetry is also smaller than that found in time-of-flight experiments. Fine structure is apparent in two different representations of the data. The energy spectrum of heavy fragments in coincidence with light fragment energies is greater than the most probable value. This structure becomes more pronounced as the light fragment energy increases. The mass yield curves for a given total kinetic energy show a structure suggesting a preference for fission fragments with masses ∼134, ∼140 and ∼145 (and their light fragment partners). Much of the structure observed can be understood by considering a semi-empirical mass surface and a simple model for the nuclear configuration at the saddle point. (author) [fr
Neutron induced fission of U isotopes up to 100 MeV
International Nuclear Information System (INIS)
Lestone, J.P.; Gavron, A.
1993-01-01
We have developed a statistical model description of the neutron induced fission of U isotopes using densities of intrinsic states and spin cut off parameters obtained directly from appropriate Nilsson model single particle levels. The first chance fission cross sections are well reproduced when the rotational contributions to the nuclear level densities are taken into account. In order to fit the U(n,f) cross sections above the threshold of second chance fission, we need to: (1) assume that the triaxial level density enhancement is washed out at an excitation energy of ∼7 MeV above the triaxial barriers with a width of ∼1 MeV, implying a γ deformation for the first barriers of 10 degree < γ < 20 degree; and (2) include pre-equilibrium particle emission in the calculations. Above an incoming neutron kinetic energy of ∼17 MeV our statistical model U(n,f) cross sections increasingly overestimate the experimental data when so called ''good'' optical model potentials are used to calculate the compound nucleus formation cross sections. This is not surprising since at these high energies little data exists on the scattering of neutrons to help guide the choice of optical model parameters. A satisfactory reproduction of all the available U(n,f) cross sections above 17 MeV is obtained by a simple scaling of our calculated compound nucleus formation cross sections. This scaling factor falls from 1.0 at 17 MeV to 0.82 at 100 MeV
On Use of Multi-Chambered Fission Detectors for In-Core, Neutron Spectroscopy
Roberts, Jeremy A.
2018-01-01
Presented is a short, computational study on the potential use of multichambered fission detectors for in-core, neutron spectroscopy. Motivated by the development of very small fission chambers at CEA in France and at Kansas State University in the U.S., it was assumed in this preliminary analysis that devices can be made small enough to avoid flux perturbations and that uncertainties related to measurements can be ignored. It was hypothesized that a sufficient number of chambers with unique reactants can act as a real-time, foilactivation experiment. An unfolding scheme based on maximizing (Shannon) entropy was used to produce a flux spectrum from detector signals that requires no prior information. To test the method, integral, detector responses were generated for singleisotope detectors of various Th, U, Np, Pu, Am, and Cs isotopes using a simplified, pressurized-water reactor spectrum and fluxweighted, microscopic, fission cross sections, in the WIMS-69 multigroup format. An unfolded spectrum was found from subsets of these responses that had a maximum entropy while reproducing the responses considered and summing to one (that is, they were normalized). Several nuclide subsets were studied, and, as expected, the results indicate inclusion of more nuclides leads to better spectra but with diminishing improvements, with the best-case spectrum having an average, relative, group-wise error of approximately 51%. Furthermore, spectra found from minimum-norm and Tihkonov-regularization inversion were of lower quality than the maximum entropy solutions. Finally, the addition of thermal-neutron filters (here, Cd and Gd) provided substantial improvement over unshielded responses alone. The results, as a whole, suggest that in-core, neutron spectroscopy is at least marginally feasible.
Calculation of neutron importance function in fissionable assemblies using Monte Carlo method
International Nuclear Information System (INIS)
Feghhi, S. A. H.; Afarideh, H.; Shahriari, M.
2007-01-01
The purpose of the present work is to develop an efficient solution method to calculate neutron importance function in fissionable assemblies for all criticality conditions, using Monte Carlo Method. The neutron importance function has a well important role in perturbation theory and reactor dynamic calculations. Usually this function can be determined by calculating adjoint flux through out solving the Adjoint weighted transport equation with deterministic methods. However, in complex geometries these calculations are very difficult. In this article, considering the capabilities of MCNP code in solving problems with complex geometries and its closeness to physical concepts, a comprehensive method based on physical concept of neutron importance has been introduced for calculating neutron importance function in sub-critical, critical and supercritical conditions. For this means a computer program has been developed. The results of the method has been benchmarked with ANISN code calculations in 1 and 2 group modes for simple geometries and their correctness has been approved for all three criticality conditions. Ultimately, the efficiency of the method for complex geometries has been shown by calculation of neutron importance in MNSR research reactor
Reliability of Monte Carlo simulations in modeling neutron yields from a shielded fission source
Energy Technology Data Exchange (ETDEWEB)
McArthur, Matthew S., E-mail: matthew.s.mcarthur@gmail.com; Rees, Lawrence B., E-mail: Lawrence_Rees@byu.edu; Czirr, J. Bart, E-mail: czirr@juno.com
2016-08-11
Using the combination of a neutron-sensitive {sup 6}Li glass scintillator detector with a neutron-insensitive {sup 7}Li glass scintillator detector, we are able to make an accurate measurement of the capture rate of fission neutrons on {sup 6}Li. We used this detector with a {sup 252}Cf neutron source to measure the effects of both non-borated polyethylene and 5% borated polyethylene shielding on detection rates over a range of shielding thicknesses. Both of these measurements were compared with MCNP calculations to determine how well the calculations reproduced the measurements. When the source is highly shielded, the number of interactions experienced by each neutron prior to arriving at the detector is large, so it is important to compare Monte Carlo modeling with actual experimental measurements. MCNP reproduces the data fairly well, but it does generally underestimate detector efficiency both with and without polyethylene shielding. For non-borated polyethylene it underestimates the measured value by an average of 8%. This increases to an average of 11% for borated polyethylene.
Neutron capture cross-section of fission products in the European activation file EAF-3
International Nuclear Information System (INIS)
Kopecky, J.; Delfini, M.G.; Kamp, H.A.J. van der; Gruppelaar, H.; Nierop, D.
1992-05-01
This paper contains a description of the work performed to extend and revise the neutron capture data in the European Activation File (EAF-3) with emphasis on nuclides in the fission-product mass range. The starter was the EAF-1 data file from 1989. The present version, EAF/NG-3, contains (n,γ) excitation functions for all nuclides (729 targets) with half-lives exceeding 1/2 day in the mass range from H-1 to Cm-248. The data file is equipped with a preliminary uncertainty file, that will be improved in the near future. (author). 19 refs.; 5 figs.; 3 tabs
Liquid metal coolants for fusion-fission hybrid system: A neutronic analysis
Energy Technology Data Exchange (ETDEWEB)
Marques, Renato V.A.; Velasquez, Carlos E.; Pereira, Claubia; Veloso, Maria Auxiliadora F.; Costa, Antonella L., E-mail: claubia@nuclear.ufmg.br [Universidade de Minas Gerais (UFMG), Belo Horizonte, MG (Brazil). Departamento de Engenharia Nuclear; Barros, Graiciany P. [Comissão Nacional de Energia Nuclear (CNEN), Rio de Janeiro, RJ (Brazil)
2017-07-01
Based on a work already published by the UFMG Nuclear Engineering Department, it was suggested to use different coolant materials in a fusion-fission system after a fuel burnup simulation, including that one used in reference work. The goal is to compare the neutron parameters, such as the effect multiplication factor and actinide amounts in transmutation layer, for each used coolant and find the best(s) coolant material(s) to be applied in the considered system. Results indicate that the lead and lead-bismuth coolant are the most suitable choices to be applied to cool the system. (author)
Life shortening, tumor induction, and tissue dose for fission-neutron and gamma-ray irradiations
International Nuclear Information System (INIS)
Grahn, D.; Duggal, K.; Lombard, L.S.
1985-01-01
The primary focus of this program is to obtain information on the late effects of whole body exposure to low doses of a high linear-energy-transfer (LET) and a low-LET ionizing radiation in experimental animals to provide guidance for the prediction of radiation hazards to man. The information obtained takes the form of dose-response curves for life shortening and for the induction of numerous specific types of tumors. The animals are irradiated with fission neutrons from the Janus reactor and with 60 Co gamma rays, delivered as single, weekly, or duration-of-life exposures covering the range of doses and dose rates. 6 refs
Experimental study of a methodology for Fission-track Dating without neutron irradiation
International Nuclear Information System (INIS)
Hadler, J.C.; Iunes, P.J.; Tello, C.A.; Chemale, F.; Kawashita, K.; Curvo, E.A.C.; Santos, F.G.S.; Gasparini, T.E.; Moreira, P.A.F.P.; Guedes, S.
2009-01-01
To carry out the dating by the Fission Track Method (FTM) the international community that works with this method employs methodologies in which the mineral to be dated must be irradiated with neutrons. Such irradiation, performed in a nuclear reactor, demand a relatively long waiting time so that the activity of the sample attain a proper level for handling. The present work aims to establish a methodology that makes possible the dating by FTM using a mass spectrometer instead of a nuclear reactor. This methodology was applied to apatite samples from Durango, Mexico.
In-reactor testing of self-powered neutron detectors and miniature fission chambers
International Nuclear Information System (INIS)
Duchene, J.; LeMeur, R.; Verdant, R.
1975-01-01
The CEA has tested a variety of ''slow'' self-powered neutron detectors with rhodium, silver and vanadium emitters. Currently there are 120 vanadium detectors in the EL4 heavy water reactor. In addition, ''fast'' detectors with cobalt emitters have been tested at Saclay and 50 of these are in reactor. Other studies are concerned with 6 mm diameter miniature fission chambers. Two fast response chambers with argon-nitrogen filling gas became slow during irradiation, but operated to 600 deg C. An argon filled chamber of 4.7 mm diameter, for traversing in core system in pressurized water reactor, has shown satisfactory test results. (author)
Monte-Carlo Generation of Time Evolving Fission Chains
Energy Technology Data Exchange (ETDEWEB)
Verbeke, Jerome M. [Lawrence Livermore National Lab. (LLNL), Livermore, CA (United States); Kim, Kenneth S. [Lawrence Livermore National Lab. (LLNL), Livermore, CA (United States); Prasad, Manoj K. [Lawrence Livermore National Lab. (LLNL), Livermore, CA (United States); Snyderman, Neal J. [Lawrence Livermore National Lab. (LLNL), Livermore, CA (United States)
2013-08-01
About a decade ago, a computer code was written to model neutrons from their “birth” to their final “death” in thermal neutron detectors (^{3}He tubes): SrcSim had enough physics to track the neutrons in multiplying systems, appropriately increasing and decreasing the neutron population as they interacted by absorption, fission and leakage. The theory behind the algorithms assumed that all neutrons produced in a fission chain were all produced simultaneously, and then diffused to the neutron detectors. For cases where the diffusion times are long compared to the fission chains, SrcSim is very successful. Indeed, it works extraordinarily well for thermal neutron detectors and bare objects, because it takes tens of microseconds for fission neutrons to slow down to thermal energies, where they can be detected. Microseconds are a very long time compared to the lengths of the fission chains. However, this inherent assumption in the theory prevents its use to cases where either the fission chains are long compared to the neutron diffusion times (water-cooled nuclear reactors, or heavily moderated object, where the theory starts failing), or the fission neutrons can be detected shortly after they were produced (fast neutron detectors). For these cases, a new code needs to be written, where the underlying assumption is not made. The purpose of this report is to develop an algorithm to generate the arrival times of neutrons in fast neutron detectors, starting from a neutron source such as a spontaneous fission source (^{252}Cf) or a multiplying source (Pu). This code will be an extension of SrcSim to cases where correlations between neutrons in the detectors are on the same or shorter time scales as the fission chains themselves.
International Nuclear Information System (INIS)
Damask, A.C.; Van Konynenburg, R.; Borg, R.J.; Dienes, G.J.
1976-01-01
Enhancement of substitutional diffusion is observed in α brass (30 wt% Zn) by following the decrease in electrical resistivity with neutron irradiation of a thermally equilibrated alloy; the decrease arises from the increase in short-range order. It was determined by previous research that this diffusion enhancement is largely caused by the annealling of radiation-produced vacancies in excess of the thermal equilibrium concentration. Therefore, the results reported here are based upon a well-established technique. The rate of resistivity change per neutron of different energies will give the relative number of free vacancies produced per neutron. This experiment compares the effect of 14.8 MeV neutrons with neutrons from a fission reactor. The results indicate that 14.8 MeV neutrons produce 10 +- 2 times as many free vacancies as reactor neutrons when the latter are expressed in terms of those neutrons with energies greater than 0.1 MeV. (author)
On accelerator neutron/γ-ray incineration of long-lived fission products
International Nuclear Information System (INIS)
Nakamura, H.
1995-01-01
A methodology for evaluation and control of the incineration of Long-Lived Fission Products (LLFPs) by using the accelerator neutrons/γ-rays is presented. An arbitrary number of the auxiliary transmutation chains, each of which consists of a LLFP and its reaction precursors up to 144, are used for calculating the time-dependent depletion-production of the LLFP. In the energy range below 20 MeV, about 20 types of neutron reaction are energetically possible. The semi-empirical formulas and its parameter systematics are used for all the energy dependent reaction cross sections. A computer code TRANS-N.G based on the foregoing prescription for nuclear reactions could be applied to the LLFP incineration strategies under a large variety of situations. (author)
An evaluation of neutron and gamme heating in fission product isotopes
International Nuclear Information System (INIS)
Leal, L.C.; Hill, R.N.; Khalil, H.S.
1993-01-01
The accurate prediction of the energy deposition rate in fast reactors, particularly in blanket and nonfueled regions, requires explicit treatment of gamma photon transport. Such an explicit treatment is part of the coupled neutron-photon heating method in use at Argonne National Laboratory, (ANL). In applying this procedure, three approximations are made in connection with the modeling of fission products (FPs): 1. The contribution of the FP neutron interactions to the gamma source is neglected. 2. In computing the macroscopic gamma interaction cross sections, the FPs are either neglected or simulated with an element (usually molybdenum) representative of an open-quotes averageclose quotes FP. 3. The heating contribution of the FP is neglected by use of zero FP kerma factors
International Nuclear Information System (INIS)
Huiskamp, R.
1991-01-01
Radiation-induced acute myeloid leukemia (AML) in male CBA/H mice was used as a model for investigation of the effect of reduced fast fission neutron exposure rates on radiation-induced carcinogenesis. Groups of about 90 male CBA/H mice were irradiated or sham-irradiated at the age of 15-20 weeks. The animals were exposed to 400 mGy fast fission neutrons at exposure rates of 2, 10 or 100 mGy/min. The investigation clearly showed that reducing the exposure rate of high-LET fast fission neutrons had no influence on the incidence of AML or on the survival of the irradiated mice. In contrast, a higher incidence of lymphosarcomas was observed in mice irradiated with higher exposure rates. (orig./MG)
Energy Technology Data Exchange (ETDEWEB)
Huiskamp, R [Stichting Energieonderzoek Centrum Nederland, Petten (Netherlands). Radiobiology and Radio-Ecology Unit
1991-06-01
Radiation-induced acute myeloid leukemia (AML) in male CBA/H mice was used as a model for investigation of the effect of reduced fast fission neutron exposure rates on radiation-induced carcinogenesis. Groups of about 90 male CBA/H mice were irradiated or sham-irradiated at the age of 15-20 weeks. The animals were exposed to 400 mGy fast fission neutrons at exposure rates of 2, 10 or 100 mGy/min. The investigation clearly showed that reducing the exposure rate of high-LET fast fission neutrons had no influence on the incidence of AML or on the survival of the irradiated mice. In contrast, a higher incidence of lymphosarcomas was observed in mice irradiated with higher exposure rates. (orig./MG).
Simulated production rates of exotic nuclei from the ion guide for neutron-induced fission at IGISOL
Energy Technology Data Exchange (ETDEWEB)
Jansson, Kaj; Al-Adili, Ali; Nilsson, Nicklas; Norlin, Martin; Solders, Andreas [Uppsala University, Department of Physics and Astronomy, Uppsala (Sweden)
2017-12-15
An investigation of the stopping efficiency of fission products, in the new ion guide designed for ion production through neutron-induced fission at IGISOL in Jyvaeskylae, Finland, has been conducted. Our simulations take into account the new neutron converter, enabling measurements of neutron-induced fission yields, and thereby provide estimates of the obtained yields as a function of primary proton beam current. Different geometries, targets, and pressures, as well as models for the effective charge of the stopped ions were tested, and optimisations to the setup for higher yields are suggested. The predicted number of ions stopped in the gas lets us estimate the survival probability of the ions reaching the downstream measurements stations. (orig.)
Energy Technology Data Exchange (ETDEWEB)
Carlsson, Magnus
2004-06-01
Areas ranging from nuclear structure models to accelerator-driven systems benefit from improved neutron-induced fission data in the intermediate energy region. In this Master's degree thesis, the fragment angular distribution from fission of {sup 238}U, induced by 21-MeV neutrons, has been analysed from an experiment performed with the Medley/DIFFICILE setup at the The Svedberg Laboratory in Uppsala. The data have been corrected for low energy neutrons in the beam. The results agree with other experiments, as well as with model calculations. The data should be a starting point for further analysis with a goal to deduce the fission cross-section of {sup 238}U.
Romanets, Y; Vaz, P; Herrera-Martinez, A; Kadi, Y; Kharoua, C; Lettry, J; Lindroos, M
The EURISOL (The EURopean Isotope Separation On-Line Radioactive Ion Beam) project aims at producing high intensity radioactive ion beams produced by neutron induced fission on a fissile target (235U) surrounding a liquid mercury converter. A proton beam of 1 GeV and 4 MW impinges on the Hg converter generating by spallation reactions high neutron fluxes. In this work the state-of-the-art Monte Carlo codes MCNPX and FLUKA were used to assess the neutronics performance of the system which geometry, inspired from the MAFF concept, allows a versatile manipulation of the fission targets. The objective of the study was to optimize the geometry of the system and the materials used in the fuel and reflector elements of the system, in order to achieve the highest possible fission rate.
AUS, Neutron Transport and Gamma Transport System for Fission Reactors and Fusion Reactors
International Nuclear Information System (INIS)
1990-01-01
1 - Description of program or function: AUS is a neutronics code system which may be used for calculations of a wide range of fission reactors, fusion blankets and other neutron applications. The present version, AUS98, has a nuclear cross section library based on ENDF/B-VI and includes modules which provide for reactor lattice calculations, one-dimensional transport calculations, multi-dimensional diffusion calculations, cell and whole reactor burnup calculations, and flexible editing of results. Calculations of multi-region resonance shielding, coupled neutron and photon transport, energy deposition, fission product inventory and neutron diffusion are combined within the one code system. The major changes from the previous release, AUS87, are the inclusion of a cross-section library based on ENDF/B-VI, the addition of the POW3D multi-dimensional diffusion module, the addition of the MICBURN module for controlling whole reactor burnup calculations, and changes to the system as a consequence of moving from IBM mainframe computers to UNIX workstations. 2 - Method of solution: AUS98 is a modular system in which the modules are complete programs linked by a path given in the input stream. A simple path is simply a sequence of modules, but the path is actually pre-processed and compiled using the Fortran 77 compiler. This provides for complex module linking if required. Some of the modules included in AUS98 are: MIRANDA Cross-section generation in a multi-region resonance subgroup calculation and preliminary group condensation. ANAUSN One-dimensional discrete ordinates calculation. ICPP Isotropic collision probability calculation in one dimension and for rod clusters. POW3D Multi-dimensional neutron diffusion calculation including feedback-free kinetics. AUSIDD One-dimensional diffusion calculation. EDITAR Reaction-rate editing and group collapsing following a transport calculation. CHAR Lattice and global burnup calculation. MICBURN Control of global burnup
Independent yields of Rb and Cs isotopes from thermal-neutron induced fission of /sup 235/U
Energy Technology Data Exchange (ETDEWEB)
Balestrini, S.J.; Decker, R.; Wollnik, H.; Wuensch, K.D.; Jung, G.; Koglin, E.; Siegert, G.
1979-12-01
The relative yields of Rb and Cs isotopes from thermal-neutron fission of /sup 235/U have been redetermined using the mass separator OSTIS, on-line at a neutron guide of the High-Flux Beam Reactor at the Institut Laue-Langevin, Grenoble, France. The separator ion source was a hot oven containing /sup 235/U in a graphite matrix. The neutron beam was pulsed. Alkali fission products diffused out of the graphite and were ionized, thus producing a stepwise increase in the analyzed ion beam proportional to the independent fission yield. The ion beam and the fissions in the source were monitored simultaneously. The diffusion of Rb and Cs from the source was exponential in time with half-lives ranging from 2.8 to 18 sec, depending upon the element and source temperature. The independent fission yields of Rb and Cs are normalized by equating their element yields to each other and to a value computed from the charge distributions observed with the recoil separator LOHENGRIN and well established mass yields. Fractional independent yields are deduced from the independent fission yields, and these compare very well with the EOZ model described by Wahl.
International Nuclear Information System (INIS)
Schriewer, J.; Hehn, G.; Mattes, M.; Pfister, G.; Keinert, J.
1978-01-01
Calculations were made for different benchmark experiments in order to test the coupled multigroup neutron and gamma library EURLIB-3 with 100 neutron groups and 20 gamma groups. In cooperation with EURATOM, Ispra, we produced this shielding library recently from ENDF/B-IV data for application in fission and fusion technology. Integral checks were performed for natural lithium, carbon, oxygen, and iron. Since iron is the most important structural material in nuclear technology, we started with calculations of iron benchmark experiments. Most of them are integral experiments of INR, Karlsruhe, but comparisons were also done with benchmark experiments from USA and Japan. For the experiments with fission sources we got satisfying results. All details of the resonances cannot be checked with flux measurements and multigroup cross sections used. But some averaged resonance behaviour of the measured and calculated fluxes can be compared and checked within the error limits given. We get greater differences in the calculations of benchmark experiments with 14 MeV neutron sources. For iron the group cross sections of EURLIB-3 produce an underestimation of the neutron flux in a broad energy region below the source energy. The conclusion is that the energy degradation by inelastic scattering is too strong. For fusion application the anisotropy of the inelastic scatter process must be taken into account, which isn't done by the processing codes at present. If this effect isn't enough, additional corrections have to be applied to the inelastic cross sections of iron in ENDF/B-IV. (author)
International Nuclear Information System (INIS)
Ruddy, F.H.
1988-01-01
A method for producing a fissionable deposit of selectively ultralow mass for neutron dosimetry is described comprising the steps of: (a) spacing in opposing relation a substrate and an alpha-emitting parent source which decays to implant into the substrate of fissionable daughter ejected from the parent source as a result of the decay; and (b) holding the opposing relation for a period of time until the parent source decays to form a corresponding mass of isotopically pure fissionable daughter uniformly on the substrate
Energy Technology Data Exchange (ETDEWEB)
Frame, Katherine Chiyoko [Los Alamos National Lab. (LANL), Los Alamos, NM (United States)
2017-06-28
Neutron multiplicity measurements are widely used for nondestructive assay (NDA) of special nuclear material (SNM). When combined with isotopic composition information, neutron multiplicity analysis can be used to estimate the spontaneous fission rate and leakage multiplication of SNM. When combined with isotopic information, the total mass of fissile material can also be determined. This presentation provides an overview of this technique.
Energy Technology Data Exchange (ETDEWEB)
Mukerji, Sadhana; Krishnani, Pritam Das; Suryanarayana, Saraswatula Venkat; Naik, Haladhara; Goswami, Ashok [Bhabha Atomic Research Centre, Mumbai (India); Shivashankar, Byrapura Siddaramaiah [Manipal University, Manipal (India); Mulik, Vikas Kaluram [University of Pune, Pune (India)
2014-07-15
The yields of various fission products in the neutron-induced fission of {sup 238}U with the flux-weighted averaged neutron energies of 9.35 MeV and 12.52 MeV were determined by using an off-line gamma ray spectroscopic technique. The neutrons were generated using the {sup 7}Li(p, n) reaction at Bhabha Atomic Research Centre-Tata Institute of Fundamental Research Pelletron facility, Mumbai. The gamma- ray activities of the fission products were counted in a highly-shielded HPGe detector over a period of several weeks to identify the decaying fission products. At both the neutron energies, the fission-yield values are reported for twelve fission product. The results obtained from the present work have been compared with the similar data for mono-energetic neutrons of comparable energy from the literature and are found to be in good agreement. The peak-to-valley (P/V) ratios were calculated from the fission-yield data and were found to decreases for neutron energy from 9.35 to 12.52 MeV, which indicates the role of excitation energy. The effect of the nuclear structure on the fission product-yield is discussed.
Mukerji, Sadhana; Krishnani, Pritam Das; Shivashankar, Byrapura Siddaramaiah; Mulik, Vikas Kaluram; Suryanarayana, Saraswatula Venkat; Naik, Haladhara; Goswami, Ashok
2014-07-01
The yields of various fission products in the neutron-induced fission of 238U with the flux-weightedaveraged neutron energies of 9.35 MeV and 12.52 MeV were determined by using an off-line gammaray spectroscopic technique. The neutrons were generated using the 7Li(p, n) reaction at Bhabha Atomic Research Centre-Tata Institute of Fundamental Research Pelletron facility, Mumbai. The gamma- ray activities of the fission products were counted in a highly-shielded HPGe detector over a period of several weeks to identify the decaying fission products. At both the neutron energies, the fission-yield values are reported for twelve fission product. The results obtained from the present work have been compared with the similar data for mono-energetic neutrons of comparable energy from the literature and are found to be in good agreement. The peak-to-valley (P/V) ratios were calculated from the fission-yield data and were found to decreases for neutron energy from 9.35 to 12.52 MeV, which indicates the role of excitation energy. The effect of the nuclear structure on the fission product-yield is discussed.
Spontaneous scalarization with an extremely massive field and heavy neutron stars
Morisaki, Soichiro; Suyama, Teruaki
2017-10-01
We investigate the internal structure and the mass-radius relation of neutron stars in a recently proposed scalar-tensor theory dubbed asymmetron in which a massive scalar field undergoes spontaneous scalarization inside neutron stars. We focus on the case where the Compton wavelength is shorter than 10 km, which has not been investigated in the literature. By solving the modified Einstein equations, either purely numerically or by partially using a semianalytic method, we find that not only the weakening of gravity by spontaneous scalarization but also the scalar force affect the internal structure significantly in the massive case. We also find that the maximum mass of neutron stars is larger for certain parameter sets than that in general relativity and reaches 2 M⊙ even if the effect of strange hadrons is taken into account. There is even a range of parameters where the maximum mass of neutron stars largely exceeds the threshold that violates the causality bound in general relativity.
International Nuclear Information System (INIS)
Peneliau, Y.; Litaize, O.; Archier, P.; De Saint Jean, C.
2014-01-01
A large set of nuclear data are investigated to improve the calculation predictions of the new neutron transport simulation codes. With the next generation of nuclear power plants (GEN IV projects), one expects to reduce the calculated uncertainties which are mainly coming from nuclear data and are still very important, before taking into account integral information in the adjustment process. In France, future nuclear power plant concepts will probably use MOX fuel, either in Sodium Fast Reactors or in Gas Cooled Fast Reactors. Consequently, the knowledge of 239 Pu cross sections and other nuclear data is crucial issue in order to reduce these sources of uncertainty. The Prompt Fission Neutron Spectra (PFNS) for 239 Pu are part of these relevant data (an IAEA working group is even dedicated to PFNS) and the work presented here deals with this particular topic. The main international data files (i.e. JEFF-3.1.1, ENDF/B-VII.0, JENDL-4.0, BRC-2009) have been considered and compared with two different spectra, coming from the works of Maslov and Kornilov respectively. The spectra are first compared by calculating their mathematical moments in order to characterize them. Then, a reference calculation using the whole JEFF-3.1.1 evaluation file is performed and compared with another calculation performed with a new evaluation file, in which the data block containing the fission spectra (MF=5, MT=18) is replaced by the investigated spectra (one for each evaluation). A set of benchmarks is used to analyze the effects of PFNS, covering criticality cases and mock-up cases in various neutron flux spectra (thermal, intermediate, and fast flux spectra). Data coming from many ICSBEP experiments are used (PU-SOL-THERM, PU-MET-FAST, PU-MET-INTER and PU-MET-MIXED) and French mock-up experiments are also investigated (EOLE for thermal neutron flux spectrum and MASURCA for fast neutron flux spectrum). This study shows that many experiments and neutron parameters are very sensitive to
Yields and isomeric ratio of xenon and krypton isotopes from thermal neutron fission of 235U
International Nuclear Information System (INIS)
Hsu, S.S.; Lin, J.T.; Yang, C.M.; Yu, Y.W.
1981-01-01
The experimental cumulative yields of 85 Kr/sup m/, 87 Kr, 88 Kr, 133 Xe/sup g/, 135 Xe/sup m/, and 135 Xe/sup g/ and the independent isomeric yield of 133 Xe/sup m/ in the thermal neutron fission of 235 U have been measured by the gas chromatographic method. The independent yields of 133 Xe/sup g/, 135 Xe/sup m/, and 135 Xe/sup g/ were deduced with the aid of 133 I and 135 I data. The isomeric yield ratios of 133 Xe and 135 Xe have been computed and compared with theoretical values since they have the same high spin state J = 11/2 - and low spin ground state J = 3/2 + . The influence of the shell effect on the fission isomeric yield ratio is discussed. From the measured independent yield of Xe isotopes plus the reported data, the Xe-isotopic distribution curve has been constructed. The curve is compared with the isotopic distribution curves of Xe isotopes formed in 11.5 GeV proton interactions with 238 U and Cs isotopes formed in 24 GeV proton interactions with 238 U. Upon fitting the yield curves we find that only those products with N/Z> or =1.48 fit a curve typical of a binary fission process
Energy Technology Data Exchange (ETDEWEB)
Albinsson, H [Chalmers Univ. of Technology, Goeteborg (SE)
1971-07-01
Fission gamma radiation yields as functions of the total fragment kinetic energy were obtained for 235U thermal-neutron induced fission. The fragments were detected with silicon surface-barrier detectors and the gamma radiation with a Nal(Tl) scintillator. In some of the measurements mass selection was used so that the gamma radiation could also be measured as a function of fragment mass. Time discrimination between the fission gammas and the prompt neutrons released in the fission process was employed to reduce the background. The gamma radiation emitted during different time intervals after the fission event was studied with the help of a collimator, the position of which was changed along the path of the fission fragments. Fission-neutron and gamma-ray data of previous experiments were used for comparisons of the yields, and estimates were made of the variation of the prompt gamma-ray energy with the total fragment kinetic energy
International Nuclear Information System (INIS)
Yu Runlan; Li Xueliang; Cui Anzhi; Guo Jingru; Yan Shuhen; Tang Peijia; Liu Daming
1991-07-01
A rapid radiochemical procedure for Pd separation was developed. It was the first time to use radiochemical techniques to determine 114 Pd cumulative yield (2.50 ± 0.14)% in 252 Cf spontaneous fission. The cumulative yields of (3.50 ± 0.13)% and (3.70 ± 0.11)% for 112 Pd and 113g Ag were also obtained. These are in agreement with Skovorodkin's results. The cumulative yields determined show that there is a fine-structure at light peak of mass number A = 113 in the mass distribution of 252 Cf spontaneous fission
Experimental approach to fission process of actinides
Energy Technology Data Exchange (ETDEWEB)
Baba, Hiroshi [Osaka Univ., Toyonaka (Japan). Faculty of Science
1997-07-01
From experimental views, it seems likely that the mechanism of nuclear fission process remains unsolved even after the Bohr and Weeler`s study in 1939. Especially, it is marked in respect of mass distribution in unsymmetric nuclear fission. The energy dependency of mass distribution can be explained with an assumption of 2-mode nuclear fission. Further, it was demonstrated that the symmetrical fission components and the unsymmetrical ones have different saddle and fission points. Thus, the presence of the 2-mode fission mechanism was confirmed. Here, transition in the nuclear fission mechanism and its cause were investigated here. As the cause of such transition, plausible four causes; a contribution of multiple-chance fission, disappearance of shell effects, beginning of fission following collective excitation due to GDR and nuclear phase transition were examined in the condition of excitation energy of 14.0 MeV. And it was suggested that the transition in the nuclear fission concerned might be related to phase transition. In addition, the mechanism of nuclear fission at a low energy and multi-mode hypothesis were examined by determination of the energy for thermal neutron fission ({sup 233,235}U and {sup 239}Pu) and spontaneous nuclear fission ({sup 252}Cf). (M.N.)
Measurement of the uranium-235 fission cross section over the neutron energy range 1 to 6 MeV
International Nuclear Information System (INIS)
Barton, D.M.; Diven, B.C.; Hansen, G.E.; Jarvis, G.A.; Koontz, P.G.; Smith, R.K.
1976-01-01
The ratio of the fission cross section of 235 U to the scattering cross section of 1 H was measured in the 1- to 6-MeV range using monoenergetic neutrons from a pulsed 3 H(p,n) 3 He source. In this measurement, solid-state detectors determined fission fragment and recoil proton emissions from back-to-back U(99.7%) and polyethylene disks. Timing permitted discrimination against room-scattered neutron backgrounds. Absolute values for 235 U(n,f) are obtained using the Hopkins-Breit evaluation of the hydrogen-scattering cross section
International Nuclear Information System (INIS)
Moraes, O.M.G. de.
1984-01-01
A systematic study about the registration characteristics of synthetic fused quartz 'Suprasil I' use as a detector of fission fragments under high flux of reactor neutrons and the effects of irradiation on it was performed. Fission fragments of 252 Cf, gamma radiation doses of of 60 Co up to 150 MGy, and integrated neutrons fluxes up to 10 20 n/cm 2 were used. A model to explain the effects on track registration and development characteristics of 'Suprasil I' irradiated on reactors were proposed, based on the obtained results for efficiency an for annealing. (C.G.C.) [pt
International Nuclear Information System (INIS)
Filliatre, P.; Oriol, L.; Jammes, C.; Vermeeren, L.
2008-01-01
The FNDS project aims at developing fission chambers to measure on-line the fast component of a high neutron flux (∼10 14 ncm -2 s -1 or more) with a significant thermal component. We identify with simulations the deposits of fission chambers that are best suited to this goal. We address the question of the evolution of the deposit by radiative capture and decay. A deposit of 242 Pu appears as the best choice, with a high initial sensitivity to fast neutrons only slowly degrading under irradiation. The effect of unavoidable impurities was assessed: small concentrations of 241 Pu and 239 Pu can be tolerated
Angular Distribution of Gamma Rays from the Fission of {sup 235}U Induced by 14-Mev Neutrons
Energy Technology Data Exchange (ETDEWEB)
Jeki, L.; Kluge, Gy.; Lajtai, A. [Central Research Institute for Physics, Hungarian Academy of Sciences (Hungary)
1969-12-15
Experiments are reported which were performed to study the angular distribution of the gamma radiation following fast-neutron-induced nuclear fission. The investigations were, in particular, focussed on the influence which the angular momentum imparted to the compound nucleus by the fast neutrons has on the angular distribution of the {gamma}-rays. The fission of {sup 235}U is induced by 14-MeV-energy neutrons from the T(d, n) {alpha} reaction. The fission fragments are detected by a gas-scintillation counter filled with a mixture of Ar and Ni gases, the {gamma}-rays by 5 cm x 5 cm Nal(Tl) crystal with an energy threshold of 120 keV. The intensity of the {gamma}-rays is measured at 90 Degree-Sign and 174 Degree-Sign to the direction of fragment motion. The flight times of fission neutrons and {gamma}-rays are measured with a 20-ns overlap-type time-to-pulse height converter while the background was covered simultaneously with another converter delayed with respect to the former. The signals from both converters are analysed by a multichannel analyser with divisible memory. The flight path, which is chosen to be about 70 cm, makes it possible to separate the neutron from the gamma counts. The geometry is designed to keep the direction of the outflying fission fragments nearly the same as that of the incident fast neutrons. In this way the angular momenta of the fast neutrons are normal to the flight path of the fragments. The measured gamma intensities are extrapolated to 180 Degree-Sign on a computer using Strutinski's formula n( Greek-Theta-Symbol ) {approx}1 + B sin Greek-Theta-Symbol . On transformation of the measured data from the laboratory system to the system of fragments the anisotropy is found to be A = 1(180 Degree-Sign )/l (90 Degree-Sign ) = 1.33 {+-} 0.05. The main angular momentum of fission fragments is calculated from the anisotropy as 15 h units. As compared with the thermal-neutron-induced fission the present results indicate an additional
Angular distribution of gamma rays from the fission of {sup 235}U induced by 14-MeV neutrons
Energy Technology Data Exchange (ETDEWEB)
Jeki, L; Kluge, G; Lajtai, A [Central Research Institute for Physics, Hungarian Academy of Sciences (Hungary)
1969-12-15
Experiments are reported which were performed to study the angular distribution of the gamma radiation following fast-neutron-induced nuclear fission. The investigations were, in particular, focussed on the influence which the angular momentum imparted to the compound nucleus by the fast neutrons has on the angular distribution of the {gamma}-rays. The fission of {sup 235}U is induced by 14-MeV-energy neutrons from the T(d, n) {alpha} reaction. The fission fragments are detected by a gas-scintillation counter filled with a mixture of Ar and Ni gases, the {gamma}-rays by 5 cm x 5 cm Nal(Tl) crystal with an energy threshold of 120 keV. The intensity of the {gamma}-rays is measured at 90 deg. and 174 deg. to the direction of fragment motion. The flight times of fission neutrons and {gamma}-rays are measured with a 20-ns overlap-type time-to-pulse height converter while the background was covered simultaneously with another converter delayed with respect to the former. The signals from both converters are analysed by a multichannel analyser with divisible memory. The flight path, which is chosen to be about 70 cm, makes it possible to separate the neutron from the gamma counts. The geometry is designed to keep the direction of the outflying fission fragments nearly the same as that of the incident fast neutrons. In this way the angular momenta of the fast neutrons are normal to the flight path of the fragments. The measured gamma intensities are extrapolated to 180 deg on a computer using Strutinski's formula n({theta}) {approx} 1 + B sin {theta}. On transformation of the measured data from the laboratory system to the system of fragments the anisotropy is found to be A = I(180 deg.)/I (90 deg.) = 1.33 {+-} 0.05. The main angular momentum of fission fragments is calculated from the anisotropy as 15 (h/2{pi}) units. As compared with the thermal-neutron-induced fission the present results indicate an additional contribution from the angular momentum of the compound
Electron-capture delayed fission properties of neutron-deficient einsteinium nuclei
Energy Technology Data Exchange (ETDEWEB)
Shaughnessy, Dawn A. [Univ. of California, Berkeley, CA (United States)
2000-01-01
Electron-capture delayed fission (ECDF) properties of neutron-deficient einsteinium isotopes were investigated using a combination of chemical separations and on-line radiation detection methods. ^{242}Es was produced via the ^{233}U(^{14}N,5n)^{242}Es reaction at a beam energy of 87 MeV (on target) in the lab system, and was found to decay with a half-life of 11 ± 3 seconds. The ECDF of ^{242}Es showed a highly asymmetric mass distribution with an average pre-neutron emission total kinetic energy (TKE) of 183 ± 18 MeV. The probability of delayed fission (P_{DF}) was measured to be 0.006 ± 0.002. In conjunction with this experiment, the excitation functions of the ^{233}U(^{14}N,xn)^{247-x}Es and ^{233}U^{(15N,xn)}^{248-x}Es reactions were measured for ^{243}Es, ^{244}Es and ^{245}Es at projectile energies between 80 MeV and 100 MeV.
Electron-capture delayed fission properties of neutron-deficient einsteinium nuclei
International Nuclear Information System (INIS)
Shaughnessy, Dawn A.
2000-01-01
Electron-capture delayed fission (ECDF) properties of neutron-deficient einsteinium isotopes were investigated using a combination of chemical separations and on-line radiation detection methods. 242 Es was produced via the 233 U( 14 N,5n) 242 Es reaction at a beam energy of 87 MeV (on target) in the lab system, and was found to decay with a half-life of 11 ± 3 seconds. The ECDF of 242 Es showed a highly asymmetric mass distribution with an average pre-neutron emission total kinetic energy (TKE) of 183 ± 18 MeV. The probability of delayed fission (P DF ) was measured to be 0.006 ± 0.002. In conjunction with this experiment, the excitation functions of the 233 U( 14 N,xn) 247-x Es and 233 U( 15 N,xn) 248-x Es reactions were measured for 243 Es, 244 Es and 245 Es at projectile energies between 80 MeV and 100 MeV
We propose to measure the neutron-induced capture cross section of the fissile isotope $^{235}$U using a fission tagging set-up. This new set-up has been tested successfully in 2010 and combines the n_TOF 4${\\pi}$ Total Absorption Calorimeter (TAC) with MicroMegas (MGAS) fission detectors. It has been proven that such a combination of detectors allows distinguishing with very good reliability the electromagnetic cascades from the capture reactions from dominant ${\\gamma}$-ray background coming from the fission reactions. The accurate discrimination of the fission background is the main challenge in the neutron capture cross section measurements of fissile isotopes. The main results from the measurement will be the associated capture cross section and ${\\alpha}$ ratio in the resolved (0.3-2250 eV) and unresolved (2.25-30 keV) resonance regions. According to the international benchmarks and as it is mentioned in the NEA High Priority Request List (HPRL), the 235U(n,${\\gamma}$) cross section is of utmost impo...
14. International workshop on nuclear fission physics. Proceedings
International Nuclear Information System (INIS)
2000-01-01
The meetings on nuclear fission took place 12-15 October 1998 and was organized by Institute of Physics and Power Engineering. The aim of the workshop was to present and discuss main new both theoretical and experimental results obtained in the area of nuclear fission, dynamical feature, properties of fission fragments and complementary radiation. As usual the program of the workshop was designed to cover a wide range of physical phenomena - from low energy and spontaneous fission to fission of hot rotating nuclei and multifragmentation at intermediate and high energies. Reaction induced by slow and fast neutron, light and heavy ions were discussed [ru
The neutronics studies of a fusion fission hybrid reactor using pressure tube blankets
International Nuclear Information System (INIS)
Zheng Youqi; Zu Tiejun; Wu Hongchun; Cao Liangzhi; Yang Chao
2012-01-01
In this paper, a fusion fission hybrid reactor used for energy producing is proposed based on the situation of nuclear power in China. The pressurized light water is applied as the coolant. The fuel assemblies are loaded in the pressure tubes with a modular type structure. The neutronics analysis is performed to get the suitable design and prove the feasibility. The energy multiplication and tritium self-sustaining are evaluated. The neutron load is also cared. From different candidates, the PWR spent fuel is selected as the feed fuel. The results show that the hybrid reactor can meet the expected reactor core lifetime of 5 years with 1000 MWe power output. Two ways are discussed including burning the discharged PWR spent fuel and burning the reprocessed plutonium. The energy multiplication is big enough and the tritium can be self-sustaining for both of the two ways. The neutron wall load in the operating time is kept smaller than the one of ITER. The way to use the reprocessed plutonium brings low neutron wall load, but also brings additional difficulties in operating the hybrid reactor. The way to use the discharged spent fuel is proposed to be a better choice currently.
International Nuclear Information System (INIS)
Balestrini, S.J.; Balagna, J.P.; Menlove, H.O.
1976-01-01
Two specialized neutron-sensitive detectors are described which are employed for rapid assays of fissionable elements by sensing for delayed neutrons emitted by samples after they have been irradiated in a nuclear reactor. The more sensitive of the two detectors, designed to assay for uranium in water samples, is 40% efficient; the other, designed for sediment sample assays, is 27% efficient. These detectors are also designed to operate under water as an inexpensive shielding against neutron leakage from the reactor and neutrons from cosmic rays. (Auth.)
International Nuclear Information System (INIS)
Stromswold, D.C.; Peurrung, A.J.; Reeder, P.L.; Perkins, R.W.
1996-06-01
Feasibility experiments conducted at Pacific Northwest National Laboratory demonstrate that either delayed neutrons or energetic gamma rays from short-lived fission products can be used to monitor the blending of UF 6 gas streams. A 252 Cf neutron source was used to induce 235 U fission in a sample, and delayed neutrons and gamma rays were measured after the sample moved open-quotes down-stream.close quotes The experiments used a UO 2 powder that was transported down the pipe to simulate the flowing UF 6 gas. Computer modeling and analytic calculation extended the test results to a flowing UF 6 gas system. Neutron or gamma-ray measurements made at two downstream positions can be used to indicate both the 235 U content and UF 6 flow rate. Both the neutron and gamma-ray techniques have the benefits of simplicity and long-term reliability, combined with adequate sensitivity for low-intrusion monitoring of the blending process. Alternatively, measuring the neutron emission rate from (a, n) reactions in the UF 6 provides an approximate measure of the 235 U content without using a neutron source to induce fission
International Nuclear Information System (INIS)
Hanmoto, Hidehiro; Yonezawa, Yoshihiko; Itoh, Tetsuo; Kondo, Sohei.
1992-01-01
Seeds of Haplopappus gracilis (2n=4), an annual Compositae, were soaked in water for 24 hr and then irradiated with fission neutrons from the 1-wattage reactor, UTR-KINKI, or X rays. The root tip cells were inspected at 48 hr post-irradiation for evidence of chromosome damage using micronucleus as endpoint. The frequency of neutron-induced micronuclei increased almost linearly as the dose increased up to as much as 1.2 Gy. X-ray-induced micronuclei showed an exponential dose-response relation. From dose-response data, we estimated that the dose necessary to induce micronuclei at a frequency of 5 per 1,000 cells was 1.2 Gy for neutrons and 8.6 Gy for X rays. Thus, to induce chromosome damage in the somatic cells of germinating Haplopappus seeds, fission neutrons were much more effective than X rays. (author)
Krypton and xenon in Apollo 14 samples - Fission and neutron capture effects in gas-rich samples
Drozd, R.; Hohenberg, C.; Morgan, C.
1975-01-01
Gas-rich Apollo 14 breccias and trench soil are examined for fission xenon from the decay of the extinct isotopes Pu-244 and I-129, and some samples have been found to have an excess fission component which apparently was incorporated after decay elsewhere and was not produced by in situ decay. Two samples have excess Xe-129 resulting from the decay of I-129. The excess is correlated at low temperatures with excess Xe-128 resulting from neutron capture on I-127. This neutron capture effect is accompanied by related low-temperature excesses of Kr-80 and Kr-82 from neutron capture on the bromine isotopes. Surface correlated concentrations of iodine and bromine are calculated from the neutron capture excesses.
International Nuclear Information System (INIS)
Ji Gang; Guo Yong; Luo Yisheng; Zhang Wenzhong
2001-01-01
Objective: To provide useful parameters for neutron radiotherapy, the author presents results of a Monte Carlo simulation study investigating the dosimetric characteristics of linear 252 Cf fission neutron sources. Methods: A 252 Cf fission source and tissue equivalent phantom were modeled. The dose of neutron and gamma radiations were calculated using Monte Carlo Code. Results: The dose of neutron and gamma at several positions for 252 Cf in the phantom made of equivalent materials to water, blood, muscle, skin, bone and lung were calculated. Conclusion: The results by Monte Carlo methods were compared with the data by measurement and references. According to the calculation, the method using water phantom to simulate local tissues such as muscle, blood and skin is reasonable for the calculation and measurements of dose distribution for 252 Cf
International Nuclear Information System (INIS)
Lazarev, Yu.A.; Lobanov, Yu.V.; Sagajdak, R.N.; Utenkov, V.K.; Kharitonov, Yu.P.; Shirokovskij, I.V.; Tret'yakova, S.P.; Oganessyan, Yu.Ts.
1988-01-01
By employing the 249 Cf( 4 He, 3n) and 208 Pb( 48 Ca,2n) reactions, experiments to study the stability against spontaneous fission of the nuclides 250 Fm and 254 102 as well as of the two-quasi-particle (2 q-p) K isomers 250 Fm (T 1/2 =1,8±0,1 s) and 254 102 (T 1/2 =0,28±0,04 s) have been performed. The groundstate spontaneous fission of the two nuclides has been discovered and the corresponding branching ratios b sf and partial half-lives T sf , respectively, have been determined to be: (6,9±1,0)x10 -5 , 0,83±0,15 yr for 250 Fm; (1,7±0,5)x10 -3 , (3,2±0,9)x10 4 s for 254 102. As a by-product of these studies, new data about cross sections of the 206,208 Pb( 48 Ca,xn) reactions have been obtained. Experiments designed to search for the spontaneous fission of the 2 q-p K-isometric states in 250 Fm and 254 102 have not revealed the effect in question. The lower limits of the ratios of the partial spontaneous fission half-lives for the 2 q-p K-isomeric states to those for the respective ground states, T * sf /T sf , have been established to be≥10 -1 for 250m Fm/ 250 Fm and ≥5x10 -3 for 254m 102/ 254 102. This means that the stability of the 2 q-p K-isomeric states in 250 Fm and 254 102 against spontaneous fission is practically not inferior to that of the ground states of these nuclei. In accord with the experimental findings, the theoretical estimates of T * sf /T sf made in the present paper show that, due to the influence of the specialization and blocking effects on the potential energy and the effective mass associated with fission, spontaneous fission from 2 q-p K-isomeric states cannot be facilitated but, on the contrary, should be essentially hindered compared with ground-state spontaneous fission
Energy Technology Data Exchange (ETDEWEB)
Perret, G.; Jordan, K. A. [Paul Scherrer Institut, Villigen, 5232 (Switzerland)
2011-07-01
Novel techniques to measure newly induced fissions in spent fuel after re-irradiation at low power have been developed and tested at the Proteus zero-power research reactor. The two techniques are based on the detection of high energy gamma-rays emitted by short-lived fission products and delayed neutrons. The two techniques relate the measured signals to the total fission rate, the isotopic composition of the fuel, and nuclear data. They can be combined to derive better estimates on each of these parameters. This has potential for improvement in many areas. Spent fuel characterisation and safeguard applications can benefit from these techniques for non-destructive assay of plutonium content. Another application of choice is the reduction of uncertainties on nuclear data. As a first application of the combination of the delayed neutron and gamma measurement techniques, this paper shows how to reduce the uncertainties on the relative abundances of the longest delayed neutron group for thermal fissions in {sup 235}U, {sup 239}Pu and fast fissions in {sup 238}U. The proposed experiments are easily achievable in zero-power research reactors using fresh UO{sub 2} and MOX fuel and do not require fast extraction systems. The relative uncertainties (1{sigma}) on the relative abundances are expected to be reduced from 13% to 4%, 16% to 5%, and 38% to 12% for {sup 235}U, {sup 238}U and {sup 239}Pu, respectively. (authors)
Neutron-antineutron oscillation and baryonic majoron: low scale spontaneous baryon violation
Energy Technology Data Exchange (ETDEWEB)
Berezhiani, Zurab [Universita dell' Aquila, Dipartimento delle Scienze Fisiche e Chimiche, L' Aquila (Italy); INFN, Laboratori Nazionali Gran Sasso, L' Aquila (Italy)
2016-12-15
We discuss the possibility that baryon number B is spontaneously broken at low scales, of the order of MeV or even smaller, inducing the neutron-antineutron oscillation at the experimentally accessible level. An associated Goldstone particle-baryonic majoron can have observable effects in neutron to antineutron transitions in nuclei or dense nuclear matter. By extending baryon number to an anomaly-free B - L symmetry, the baryo-majoron can be identified with the ordinary majoron associated with the spontaneous breaking of lepton number, and it can have interesting implications for neutrinoless 2β decay with the majoron emission. We also discuss the hypothesis that baryon number can be spontaneously broken by QCD itself via the six-quark condensates. (orig.)
International Nuclear Information System (INIS)
Piksajkin, V.M.; Kazakov, L.E.; Isaev, S.T.; Korolev, G.G.; Roshchenko, V.A.; Tertychnyj, R.G.
2002-01-01
Relative yield and group period of delayed neutrons induced by the 239 Pu fission in the 0.37-4.97 MeV range were measured. Comparative analysis of experimental data was conducted in terms of middle period of half-life of delayed neutron nuclei-precursors. Character and scale of changing values of delayed neutron group parameters as changing excitation energy of fission compound-nucleus have been demonstrated for the first time. Considerable energy dependence of group parameters under the neutron induced 239 Pu fission that was expressed by the decreasing middle period of half-life of nuclei-precursors by 10 % in the 2.85 eV - 5 MeV range of virgin neutrons was detected [ru
Khryachkov, Vitaly; Goverdovskii, Andrei; Ketlerov, Vladimir; Mitrofanov, Vecheslav; Sergachev, Alexei
2018-03-01
Binary fission of 232Th and 238U induced by fast neutrons were under intent investigation in the IPPE during recent years. These measurements were performed with a twin ionization chamber with Frisch grids. Signals from the detector were digitized for further processing with a specially developed software. It results in information of kinetic energies, masses, directions and Bragg curves of registered fission fragments. Total statistics of a few million fission events were collected during each experiment. It was discovered that for several combinations of fission fragment masses their total kinetic energy was very close to total free energy of the fissioning system. The probability of such fission events for the fast neutron induced fission was found to be much higher than for spontaneous fission of 252Cf and thermal neutron induced fission of 235U. For experiments with 238U target the energy of incident neutrons were 5 MeV and 6.5 MeV. Close analysis of dependence of fission fragment distribution on compound nucleus excitation energy gave us some explanation of the phenomenon. It could be a process in highly excited compound nucleus which leads the fissioning system from the scission point into the fusion valley with high probability.
Measurement and analysis of thorium fission rate in a polyethylene shell with a D-T neutron source
Energy Technology Data Exchange (ETDEWEB)
Zheng, Lei [Institute of Nuclear Physics and Chemistry, China Academy of Engineering Physics, Mianyang 621900 (China); Yang, Yiwei, E-mail: winfield1920@126.com [Institute of Nuclear Physics and Chemistry, China Academy of Engineering Physics, Mianyang 621900 (China); Liu, Zhujun [Institute of Nuclear Physics and Chemistry, China Academy of Engineering Physics, Mianyang 621900 (China); Department of Nuclear Engineering and Technology, Sichuan University, Chengdu 610065,China (China); Liu, Rong, E-mail: liurongzy@163.com [Institute of Nuclear Physics and Chemistry, China Academy of Engineering Physics, Mianyang 621900 (China); Jiang, Li; Wang, Mei [Institute of Nuclear Physics and Chemistry, China Academy of Engineering Physics, Mianyang 621900 (China)
2016-12-15
Highlights: • Associated angular dependencies of the source neutron energy and intensity was given. • Two sets of fission yields from evaluated libraries were considered and applied. • Calculated results employing ENDF/B-VII.0 agreed with the experimental ones best. • Small discrepancies exist between thorium fission cross section evaluated libraries. - Abstract: In order to validate the {sup 232}Th fission cross section, an integral experiment was carried out using the activation method in a polyethylene shell with a D-T neutron source. Thorium samples were arranged in the 0° direction to the incident D{sup +} beam. The {sup 232}Th fission rate was determined by measuring the 151.195 keV characteristic γ ray emitted from the fission fragment {sup 85m}Kr, and the experimental uncertainties were about 5.3%. MCNP calculation results employing ENDF/B-VII.0, JENDL-3.3, JENDL-4.0 libraries are in good agreement with that of experiments within uncertainties except that employing ENDF/B-VII.1 (∼6.5%). The experiment results can be used to re-evaluate the {sup 232}Th fission cross section.
NEUTRON CROSS SECTION EVALUATIONS OF FISSION PRODUCTS BELOW THE FAST ENERGY REGION
International Nuclear Information System (INIS)
OH, S.Y.; CHANG, J.; MUGHABGHAB, S.
2000-01-01
Neutron cross section evaluations of the fission-product isotopes, 95 Mo, 99 Tc, 101 Ru, 103 Rh, 105 Pd, 109 Ag, 131 Xe, 133 Cs, 141 Pr, 141 Nd, 147 Sm, 149 Sm, 150 Sm, 151 Sm, 152 Sm, 153 Eu, 155 Gd, and 157 Gd were carried out below the fast neutron energy region within the framework of the BNL-KAERI international collaboration. In the thermal energy region, the energy dependence of the various cross-sections was calculated by applying the multi-level Breit-Wigner formalism. In particular, the strong energy dependence of the coherent scattering lengths of 155 Gd and 157 Gd were determined and were compared with recent calculations of Lynn and Seeger. In the resonance region, the recommended resonance parameters, reported in the BNL compilation, were updated by considering resonance parameter information published in the literature since 1981. The s-wave and, if available, p-wave reduced neutron widths were analyzed in terms of the Porter-Thomas distribution to determine the average level spacings and the neutron strength functions. Average radiative widths were also calculated from measured values of resolved energy resonances. The average resonance parameters determined in this study were compared with those in the BNL and other compilations, as well as the ENDF/B-VI, JEF-2.2, and JENDL-3.2 data libraries. The unresolved capture cross sections of these isotopes, computed with the determined average resonance parameters, were compared with measurements, as well as the ENDF/B-VI evaluations. To achieve agreement with the measurements, in a few cases minor adjustments in the average resonance parameters were made. Because of astrophysical interest, the Maxwellian capture cross sections of these nuclides at a neutron temperature of 30 keV were computed and were compared with other compilations and evaluations
NEUTRON CROSS SECTION EVALUATIONS OF FISSION PRODUCTS BELOW THE FAST ENERGY REGION
Energy Technology Data Exchange (ETDEWEB)
OH,S.Y.; CHANG,J.; MUGHABGHAB,S.
2000-05-11
Neutron cross section evaluations of the fission-product isotopes, {sup 95}Mo, {sup 99}Tc, {sup 101}Ru, {sup 103}Rh, {sup 105}Pd, {sup 109}Ag, {sup 131}Xe, {sup 133}Cs, {sup 141}Pr, {sup 141}Nd, {sup 147}Sm, {sup 149}Sm, {sup 150}Sm, {sup 151}Sm, {sup 152}Sm, {sup 153}Eu, {sup 155}Gd, and {sup 157}Gd were carried out below the fast neutron energy region within the framework of the BNL-KAERI international collaboration. In the thermal energy region, the energy dependence of the various cross-sections was calculated by applying the multi-level Breit-Wigner formalism. In particular, the strong energy dependence of the coherent scattering lengths of {sup 155}Gd and {sup 157}Gd were determined and were compared with recent calculations of Lynn and Seeger. In the resonance region, the recommended resonance parameters, reported in the BNL compilation, were updated by considering resonance parameter information published in the literature since 1981. The s-wave and, if available, p-wave reduced neutron widths were analyzed in terms of the Porter-Thomas distribution to determine the average level spacings and the neutron strength functions. Average radiative widths were also calculated from measured values of resolved energy resonances. The average resonance parameters determined in this study were compared with those in the BNL and other compilations, as well as the ENDF/B-VI, JEF-2.2, and JENDL-3.2 data libraries. The unresolved capture cross sections of these isotopes, computed with the determined average resonance parameters, were compared with measurements, as well as the ENDF/B-VI evaluations. To achieve agreement with the measurements, in a few cases minor adjustments in the average resonance parameters were made. Because of astrophysical interest, the Maxwellian capture cross sections of these nuclides at a neutron temperature of 30 keV were computed and were compared with other compilations and evaluations.
The application of n-γ discrimination in 252Cf spontaneous neutron TOF spectra measurement
International Nuclear Information System (INIS)
Zhou Haojun; Zhang Yi; Li Jiansheng; Jin Yu; Wang Jie; Li Chunyuan
2004-01-01
The BC501 scintillator is used as a fast neutron detector. The effect that the pulse rise time method was used to discriminate γ from 252 Cf spontaneous neutron TOF spectra is studied in the experiment. A pulse rise time separation spectra of γ and 252 Cf spontaneous neuron upon 1 MeV is obtained, the n-γ separation function reaches to 4.6. When the result of pulse rise time separation coincides with the time-of-flight spectra in which the neutron energy is upon 0.5 MeV, 0.8 MeV and 1.0 MeV, comparing with the anticoincidence, γ was eliminated 99.90% at least. (authors)
Evolvement simulation of the probability of neutron-initiating persistent fission chain
International Nuclear Information System (INIS)
Wang Zhe; Hong Zhenying
2014-01-01
Background: Probability of neutron-initiating persistent fission chain, which has to be calculated in analysis of critical safety, start-up of reactor, burst waiting time on pulse reactor, bursting time on pulse reactor, etc., is an inherent parameter in a multiplying assembly. Purpose: We aim to derive time-dependent integro-differential equation for such probability in relative velocity space according to the probability conservation, and develop the deterministic code Dynamic Segment Number Probability (DSNP) based on the multi-group S N method. Methods: The reliable convergence of dynamic calculation was analyzed and numerical simulation of the evolvement process of dynamic probability for varying concentration was performed under different initial conditions. Results: On Highly Enriched Uranium (HEU) Bare Spheres, when the time is long enough, the results of dynamic calculation approach to those of static calculation. The most difference of such results between DSNP and Partisn code is less than 2%. On Baker model, over the range of about 1 μs after the first criticality, the most difference between the dynamic and static calculation is about 300%. As for a super critical system, the finite fission chains decrease and the persistent fission chains increase as the reactivity aggrandizes, the dynamic evolvement curve of initiation probability is close to the static curve within the difference of 5% when the K eff is more than 1.2. The cumulative probability curve also indicates that the difference of integral results between the dynamic calculation and the static calculation decreases from 35% to 5% as the K eff increases. This demonstrated that the ability of initiating a self-sustaining fission chain reaction approaches stabilization, while the former difference (35%) showed the important difference of the dynamic results near the first criticality with the static ones. The DSNP code agrees well with Partisn code. Conclusions: There are large numbers of