From non-linear magnetoacoustics and spin reorientation transition to magnetoelectric micro/nano-systems

Science.gov (United States)

Tiercelin, Nicolas; Preobrazhensky, Vladimir; BouMatar, Olivier; Talbi, Abdelkrim; Giordano, Stefano; Dusch, Yannick; Klimov, Alexey; Mathurin, Théo.; Elmazria, Omar; Hehn, Michel; Pernod, Philippe

2017-09-01

The interaction of a strongly nonlinear spin system with a crystalline lattice through magnetoelastic coupling results in significant modifications of the acoustic properties of magnetic materials, especially in the vicinity of magnetic instabilities associated with the spin-reorientation transition (SRT). The magnetoelastic coupling transfers the critical properties of the magnetic subsystem to the elastic one, which leads to a strong decrease of the sound velocity in the vicinity of the SRT, and allows a large control over acoustic nonlinearities. The general principles of the non-linear magneto-acoustics (NMA) will be introduced and illustrated in `bulk' applications such as acoustic wave phase conjugation, multi-phonon coupling, explosive instability of magneto-elastic vibrations, etc. The concept of the SRT coupled to magnetoelastic interaction has been transferred into nanostructured magnetoelastic multilayers with uni-axial anisotropy. The high sensitivity and the non-linear properties have been demonstrated in cantilever type actuators, and phenomena such as magneto-mechanical RF demodulation have been observed. The combination of the magnetic layers with piezoelectric materials also led to stress-mediated magnetoelectric (ME) composites with high ME coefficients, thanks to the SRT. The magnetoacoustic effects of the SRT have also been studied for surface acoustic waves propagating in the magnetoelastic layers and found to be promising for highly sensitive magnetic field sensors working at room temperature. On the other hand, mechanical stress is a very efficient way to control the magnetic subsystem. The principle of a very energy efficient stress-mediated magnetoelectric writing and reading in a magnetic memory is described.

Investigation of spin-reorientation phase transitions at surface and in volume of alpha-Fe sub 2 O sub 3 monocrystals

CERN Document Server

Kamzin, A S

2002-01-01

The magnetic structure of the surface layer and volume and the processes, observed by the spin-reorientation phase transition (SRPT), are studied in the direct comparison of the properties of the thin surface layer and the volume of the hematite (alpha-Fe sub 2 O sub 3) macroscopic crystals. The method of simultaneous gamma, X-ray and electron Moessbauer spectroscopy was used in the studies. The direct data on the existence of the transition layer on the hematite crystals surface are obtained. It is established, that the Morin-type SRPT in the sample volume occurs by a jump (the first-order phase transition). The SRPT in the surface layer as well as in the crystal volume is accompanied by formation of the intermediate state, wherein the low- and high-temperature phases coexist. The obtained experimental data on the SRPT mechanism in the surface layer agree well with the conclusions of the phenomenological theory

Extrinsic Curie temperature and spin reorientation changes in Nd2Fe14B/α-Fe nanocomposites

International Nuclear Information System (INIS)

Lewis, L.H.; Panchanathan, V.

1998-05-01

The Curie temperatures and spin reorientation temperatures of a series of four melt-spun nanocomposite materials comprised of Nd 2 Fe 1 4B and varying amounts of α-Fe were measured using independent techniques. The phase constitution and grain size was assessed with synchrotron x-ray diffraction; the Curie temperatures were measured by differential thermal analysis (DTA) and dc SQUID magnetometry in the temperature range 375 K ≤ T ≤ 800 K, whereas the spin reorientation transition temperature was determined from ac susceptibility measurements taken in the range 10 K ≤ T ≤ 300 K. The Curie temperature increases with increasing excess iron content, resulting in a 18 degree enhancement over the Curie temperature of pure Nd 2 Fe 14 B for 27 wt% excess α-Fe. The spin reorientation temperatures are depressed from the single-crystal value by an average of 10 degrees. Both anomalous effects are attributed to intergranular exchange coupling present in the alloys, although the effects of uncompensated stress between the constituent phases cannot be ruled out The experimental results suggest that while the Curie temperature of the Nd 2 Fe 14 B phase may be extrinsically enhanced significantly beyond the bulk value, possibly extending the range of applications of this compound, the anisotropy may be simultaneously lowered, impeding the attainment of high coercivities in these alloys

Dielectric resonance in ErFeO3 in the region of spin reorientation

International Nuclear Information System (INIS)

Dan'shin, N.K.; Kovtun, N.M.; Sdvizhkov, M.A.

1984-01-01

In the region of spin reorientation in ErFeO 3 in the millimetre wave range a dielectric resonance has been found - excitation of electromaqnetic field natural oscillations in spherical samples. The fregurncies of dielectric resonance in samples from ErFeO 3 possess strong independence of temperature and magnetic field in the vicinity of the spin reorientation for account of a strong growth in the magnetic susceptibility. The frequencies change most considerably in the region of low-temperature spin reorientation related to antiferromagnetic rare earth ordering. Strong anisotropy of magnetic susceptibility cases various temperature and field dependences of the dielectric resonance frequencies at different orientations of the exciting electromagnetic field relative to the crystal axes. It is shown that the method of dielectric resonance permits to determine with high accuracy the temperatures of spontaneous - and crystal fields of induced phase transformations. The crystal dielectric permittivity and magnetic permeability dispersion are determined

Effects of particle size on the spin reorientation transition in R2F14B (R=Nd, Er) hard magnets

International Nuclear Information System (INIS)

Foldeaki, M.; Koszegi, L.; Dunlap, R.A.

1991-01-01

Spin reorientation transitions (SRTs) were observed via ac-susceptibility measurements in powdered and as-cast R 2 F 14 B (R=Nd, Er) alloys. The temperature dependence of the susceptibility was found to be largely structure sensitive: powdered samples showed a moderate increase before the transition and a sharp decrease following the transition, while a sharp cusp in the susceptibility preceeded the transition in bulk samples. At the same time, the transition temperature and the relative intensity of the effects did not show any frequency dependence in the 0.1-10 kHz range. The results were compared with existing theoretical models assuming different magnetization mechanisms such as rotation of the magnetization vector, domain wall bowing and domain wall displacement. Domain wall contributions to the overall susceptibility cannot be neglected in either sample. At the same time, the rotational susceptibility is more significantly influenced by the sign reversal of the anisotropy constant, and this is the main contribution to the susceptibility maximum at the SRT. In powders, the expected sharp increase of the rotational susceptibility is counterbalanced by magnetostatic surface effects (''μ * effect''). In bulk materials the influence of surface effects is less significant and the cusp can be observed. (orig.)

Spin reorientation and structural relaxation of atomic layers: Pushing the limits of accuracy

International Nuclear Information System (INIS)

Meyerheim, H.L.; Sander, D.; Popescu, R.; Kirschner, J.; Robach, O.; Ferrer, S.

2004-01-01

The correlation between an ad-layer-induced spin reorientation transition (SRT) and the ad-layer-induced structural relaxation is investigated by combined in situ surface x-ray diffraction and magneto-optical Kerr-effect experiments on Ni/Fe/Ni(111) layers on W(110). The Fe-induced SRT from in-plane to out-of-plane, and the SRT back to in-plane upon subsequent coverage by Ni, are each accompanied by a small lattice relaxation of at most 0.002 Angstrom. Such a small strain variation excludes a magnetoelasticity driven SRT, and we suggest the interface anisotropy as a possible driving force

Spin reorientation in α-Fe2O3 nanoparticles induced by interparticle exchange interactions in alpha-Fe2O3/NiO nanocomposites

DEFF Research Database (Denmark)

Frandsen, Cathrine; Lefmann, Kim; Lebech, Bente

2011-01-01

We report that the spin structure of alpha-Fe2O3 nanoparticles rotates coherently out of the basal (001) plane at low temperatures when interacting with thin plate-shaped NiO nanoparticles. The observed spin reorientation (up to similar to 70 degrees) in alpha-Fe2O3 nanoparticles has, in appearan......, similarities to the Morin transition in bulk alpha-Fe2O3, but its origin is different-it is caused by exchange coupling between aggregated nanoparticles of alpha-Fe2O3 and NiO with different directions of easy axes of magnetization.......We report that the spin structure of alpha-Fe2O3 nanoparticles rotates coherently out of the basal (001) plane at low temperatures when interacting with thin plate-shaped NiO nanoparticles. The observed spin reorientation (up to similar to 70 degrees) in alpha-Fe2O3 nanoparticles has, in appearance...

Spin reorientation and magnetic anisotropy in Y2Co17-xCr x (x 1.17-3.0) compounds

International Nuclear Information System (INIS)

Fuquan, B.; Tegus, O.; Dagula, W.; Brueck, E.; Boer, F.R. de; Buschow, K.H.J.

2005-01-01

Spin reorientation transitions and magnetic anisotropy in Y 2 Co 17-x Cr x (x = 1.17-3.0) compounds have been investigated by means of X-ray diffraction and magnetization measurements. The powder X-ray diffraction patterns show that most samples crystallize as a single phase with the rhombohedral Th 2 Zn 17 -type structure. However, in the compound Y 2 Co 14 Cr 3 the Th 2 Zn 17 phase coexist with the hexagonal Th 2 Ni 17 -type phase. The lattice parameters a and c hardly change and the unit cell volume V increases slightly with increasing Cr content. The X-ray diffraction patterns of the aligned powder of the samples have confirmed that at room temperature the compound with x = 1.17 has planar anisotropy, but the compounds with x = 1.76, 2.34 and 3.00 have uniaxial anisotropy. Spin reorientation phenomena occur in all of the compounds. With increasing Cr content, the Curie temperature, the spin reorientation temperature, the spontaneous magnetization, and the anisotropy constant K 2 of the Y 2 Co 17-x Cr x (x = 1.17-3.0) compounds decrease strongly while the anisotropy constant K 1 increases in the range of x from 1.17 to 2.34 and then decreases in the range of x from 2.34 to 3.00

Domain structures and temperature-dependent spin reorientation transitions in c-axis oriented Co-Cr thin films

International Nuclear Information System (INIS)

Kusinski, Greg J.; Krishnan, Kannan M.; Thomas, Gareth; Nelson, E. C.

2000-01-01

Highly c-axis oriented Co 95 Cr 5 films with perpendicular anisotropy were grown epitaxially on Si (111), using an Ag seed layer, by physical vapor deposition. Films were characterized by x-ray diffraction, transmission electron microscopy (TEM), selected area electron diffraction, and Lorentz microscopy in a TEM. The following epitaxial relationship was confirmed: (111) Si (parallel sign)(111) Ag (parallel sign)(0001) CoCr ;[2(bar sign)20] Si (parallel sign)[2(bar sign)20] Ag (parallel sign)[1(bar sign)100] CoCr . Magnetic domain structures of these films were observed as a function of thickness; t, in the range, 200 Aa c ≅300 Aa, the magnetization was found to be effectively in-plane of the film, and above t c a regular, stripe-like domain pattern with a significant, alternating in sign, perpendicular component was observed. The spin reorientation transitions of the stripe domains to the in-plane magnetization were studied dynamically by observing the domains as a function of temperature by in situ heating up to 350 degree sign C. The critical transition thickness, t c , which is a function of K u and magnetostatic energy, was found to increase with increasing temperature. The stripe-domain period, L observed at room temperature was found to increase gradually with thickness; L=90 nm at t=300 Aa, and L=110 nm at t=700 Aa. (c) 2000 American Institute of Physics

Influence of the spin reorientation transition on the hysteresis characteristics of Nd-Fe-B film and bulk magnets

International Nuclear Information System (INIS)

Lileev, A.S.; Parilov, A.A.; Reissner, M.; Steiner, W.

2004-01-01

A comparison was made of the hysteresis characteristics of hard magnetic films with those of bulk samples based on Nd 2 Fe 14 B in the temperature range between 4.2 and 293 K. In both types of specimens characteristic 'dips' appear below 135 K in the demagnetisation curves which are caused by both the spin reorientation from easy axis to easy cone and the deviation from a perfect texture of the sample

Magnetostriction anisotropy in the rare earth RCo5 compounds on spontaneous spin-orientation phase transitions

International Nuclear Information System (INIS)

Ahdreev, A.V.; Deryagin, A.V.; Zadvorkin, S.M.

1983-01-01

The temperature dependences of parameters a and c in the crystal lattice of RCo 5 compounds (R=Pr, Tb, Dy, Ho) are studied in an X-ray diffractometer the spin reorientation region. On the basis of these data the magnetostriction constants lambdasub(1)sup(α, 2) and lambdasub(2)sup(α, 2) are determined for temperatures corresponding to the middle of reorientation regions of the compounds mentioned above (excluding PrCo 5 ). The values of lambdasub(1)sup(α, 2) and lambdasub(2)sup(α, 2) at T=0 K are calculated on the basis of the single-ion model for all the compounds investigalted and also for some other intermetallides of the RCo 5 type in which spontaneous spin reorien tation transitions do not occur

Exploring the dynamics about the glass transition by muon spin relaxation and muon spin rotation

International Nuclear Information System (INIS)

Bermejo, F J; Bustinduy, I; Cox, S F J; Lord, J S; Cabrillo, C; Gonzalez, M A

2006-01-01

The capability of muon spin rotation and muon spin relaxation to explore dynamics in the vicinity of the glass transition is illustrated by results pertaining to three materials exhibiting two different glass-forming abilities. Measurements under transverse magnetic fields enable us to monitor the dynamics of muonium-labelled closed-shell molecules within the microsecond range. The results display the onset of stochastic molecular motions taking place upon crossing from below the glass-transition temperature. In turn, the molecular dynamics of radicals formed by addition of atomic muonium to unsaturated organic molecules can also be explored up to far shorter times by means of relaxation measurements under longitudinal fields. The technique is then shown to be capable of singling out stochastic reorientational motions from others, which usually are strongly coupled to them and usually dominate the material response when measured using higher-frequency probes such as neutron and light scattering

Description of spin reorientation transition in Au/Co/Au sandwich with Co film thickness within a simple phenomenological model of ferromagnetic film

International Nuclear Information System (INIS)

Popov, A.P.

2012-01-01

Simple phenomenological model of ferromagnetic film characterized by equal energies of surface anisotropies at two sides of a film (symmetric film) is considered. The model is used to describe a two-step spin reorientation transition (SRT) in Au/Co/Au sandwich with Co film thickness: the SRT from perpendicular to canted noncollinear (CNC) state at N ⊥ =6.3 atomic layers and the subsequent SRT from CNC to in-plane state at N ∥ =10.05 atomic layers. Analytic expressions for the stability criterion of collinear perpendicular and in-plane states of a film are derived with account of discrete location of atomic layers. The dependence of borders that separate regions corresponding to various magnetic states of a film in the (k B ,k S )-diagram on film thickness N is established. k S (k B ) is surface (bulk) reduced anisotropy constant. The comparison of theory with experiment related to Au/Co/Au sandwich shows that there is a whole region in the (k B ,k S )-diagram corresponding to experimentally determined values of threshold film thicknesses N ⊥ =6.3 and N ∥ =10.05. The comparison of this region with similar region determined earlier for a bare Co/Au film within the same model of asymmetric film and characterized by N ⊥ =3.5, N ∥ =5.5 shows that the intersection of these regions is not empty. Hence, both the SRT in Au/Co/Au sandwich and in bare Co/Au film with Co film thickness can be described within the same model using the same magnitudes of model parameters k S , k B . Based on this result we conclude that the energy of Neel surface anisotropy at free Co surface is negligible compared to the energy of Co–Au interface anisotropy. It is demonstrated that the destabilization of collinear states in symmetric film leads to occurrence of the ground CNC state and two novel metastable CNC states. These three CNC states exhibit different kinds of symmetry. In case of asymmetric film only ground CNC state occurs on destabilization of collinear states of a film

Spin reorientation and giant low-temperature magnetostriction of polycrystalline NdFe1.9 compound

Science.gov (United States)

Tang, Y. M.; He, Y.; Huang, Y.; Zhang, L.; Tang, S. L.; Du, Y. W.

2018-04-01

The spin reorientation and magnetostriction of polycrystalline NdFe1.9 cubic Laves phase compound were investigated. A prominent transition from tetragonal symmetry to orthorhombic symmetry in NdFe1.9 compound was determined by X-ray crystallographic study. Meanwhile, a large spontaneous magnetostriction λ111 of ∼3100 ppm was detected at 15 K, which is larger than the theoretical value of 2000 ppm predicted by single-ion model. NdFe1.9 exhibits larger low-field magnetostriction than PrFe1.9 and TbFe1.9 at 5 K in the magnetic field range of H ≤ 13 kOe, which makes it a promising material for low-temperature applications. The present work might be helpful to discover inexpensive Nd-based high-performance magnetostrictive and even magnetoelectric materials for low-temperature applications.

Ferroelectricity and magnetoelectric coupling in h-YbMnO{sub 3}: Spin reorientation and defect effect

Energy Technology Data Exchange (ETDEWEB)

Qiang, Gang; Fang, Yifei; Lu, Xiaowen; Cao, Shixun; Zhang, Jincang, E-mail: jczhang@shu.edu.cn [Materials Genome Institute and Department of Physics, Shanghai University, Shanghai 200444 (China)

2016-01-11

Low-temperature magnetic and electric properties in hexagonal multiferroic compound YbMnO{sub 3} were studied. The Mn{sup 3+} spin moments order at T{sub N} = 85 K and reoriented around 43.5 K, leading to the magnetic phase transition from B{sub 2}(P6{sub 3}cm) → A{sub 2}(P6{sub 3}cm). The concomitant ferroelectric polarization is observed and explained microscopically by the destruction of initial symmetric relationship of the polarization between the upper and lower half of the magnetic unit cell. The asymmetry of the polarization vs temperature curves under opposite poling voltage revealed the pinning effect of the defects on the electrical polarization.

Superconducting spin valves controlled by spiral re-orientation in B20-family magnets

Science.gov (United States)

Pugach, N. G.; Safonchik, M.; Champel, T.; Zhitomirsky, M. E.; Lähderanta, E.; Eschrig, M.; Lacroix, C.

2017-10-01

We propose a superconducting spin-triplet valve, which consists of a superconductor and an itinerant magnetic material, with the magnet showing an intrinsic non-collinear order characterized by a wave vector that may be aligned in a few equivalent preferred directions under the control of a weak external magnetic field. Re-orienting the spiral direction allows one to controllably modify long-range spin-triplet superconducting correlations, leading to spin-valve switching behavior. Our results indicate that the spin-valve effect may be noticeable. This bilayer may be used as a magnetic memory element for cryogenic nanoelectronics. It has the following advantages in comparison to superconducting spin valves proposed previously: (i) it contains only one magnetic layer, which may be more easily fabricated and controlled; (ii) its ground states are separated by a potential barrier, which solves the "half-select" problem of the addressed switch of memory elements.

Magnetooptical studies on spin-reorientation in rare earth orthoferrites

International Nuclear Information System (INIS)

Koshizuka, N.; Hayashi, K.; Suzuki, M.; Tsushima, T.

1976-01-01

Several types of spin-reorientation (SR) in some of the RFeO 3 are studied by Faraday rotation measurements; rotational SR of GAMMA 4 → GAMMA 2 type in (ErSm)FeO 3 , (Co 2+ , Ti 4+ ) doped YFeO 3 , and abrupt SR of GAMMA 4 → GAMMA 1 type in DyFeO 3 . Observations of SR by Faraday rotation were made in these crystals with incident light parallel to the optical axis. In relation with the decrease of Fe 3+ ion's anisotropy at T/sub SR/, an abrupt decrease of the coercive force are found in these systems. In general, Faraday rotation in RFeO 3 originates from Fe 3+ ions in the visible and near IR regions, while R 3+ ion's contribution to the Faraday rotation was observed for the wavelengths corresponding to the electronic transitions of R 3+ ions in ErFeO 3 and DyFeO 3 at low temperatures. In DyFeO 3 , a large contribution of Dy 3+ ions was observed at approximately 1.2 μm in the Faraday spectrum, and it is confirmed that the Dy 3+ moments are polarized along the c-axis in zero applied field above T/sub SR/. Magnetic field induced SR was also observed in DyFeO 3 , and the temperature dependence of the critical field was obtained as H/sub SR/ varies as absolute value T - T/sub SR/3/4

Macroscopic Magnetization Control by Symmetry Breaking of Photoinduced Spin Reorientation with Intense Terahertz Magnetic Near Field

Science.gov (United States)

Kurihara, Takayuki; Watanabe, Hiroshi; Nakajima, Makoto; Karube, Shutaro; Oto, Kenichi; Otani, YoshiChika; Suemoto, Tohru

2018-03-01

We exploit an intense terahertz magnetic near field combined with femtosecond laser excitation to break the symmetry of photoinduced spin reorientation paths in ErFeO3 . We succeed in aligning macroscopic magnetization reaching up to 80% of total magnetization in the sample to selectable orientations by adjusting the time delay between terahertz and optical pump pulses. The spin dynamics are well reproduced by equations of motion, including time-dependent magnetic potential. We show that the direction of the generated magnetization is determined by the transient direction of spin tilting and the magnetic field at the moment of photoexcitation.

Detection of unusual spin reorientation induced by magnetic field in DyFeO3

International Nuclear Information System (INIS)

Balbashov, A.M.; Marchukov, P.Yu.; Nikolaev, I.V.; Rudashevskij, E.G.

1988-01-01

It is detected that in DyFeO 3 the vector of antiferromagnetism reorientates continuously in two mutually perpendicular planes, and transition from one plane into the other one is a first-order phase transformation

Temperature-induced spin reorientation and magnetization jump of rare-earth orthoferrite Ho{sub 0.5}Pr{sub 0.5}FeO{sub 3} single crystal

Energy Technology Data Exchange (ETDEWEB)

Wang, Guohua; Zhao, Weiyao; Cao, Yiming; Kang, Baojuan [Department of Physics, and International Center of Quantum and Molecular Structures, Shanghai University, Shanghai 200444 (China); Zhang, Jincang [Department of Physics, and International Center of Quantum and Molecular Structures, Shanghai University, Shanghai 200444 (China); Materials Genome Institute, Shanghai University, Shanghai 200444 (China); Shanghai Key Laboratory of High Temperature Superconductors, Shanghai University, Shanghai 200444 (China); Ren, Wei, E-mail: renwei@shu.edu.cn [Department of Physics, and International Center of Quantum and Molecular Structures, Shanghai University, Shanghai 200444 (China); Materials Genome Institute, Shanghai University, Shanghai 200444 (China); Shanghai Key Laboratory of High Temperature Superconductors, Shanghai University, Shanghai 200444 (China); Cao, Shixun, E-mail: sxcao@shu.edu.cn [Department of Physics, and International Center of Quantum and Molecular Structures, Shanghai University, Shanghai 200444 (China); Materials Genome Institute, Shanghai University, Shanghai 200444 (China); Shanghai Key Laboratory of High Temperature Superconductors, Shanghai University, Shanghai 200444 (China)

2016-07-25

We report temperature-induced spin reorientation and magnetization jump effects in the rare earth (RE) orthoferrite Ho{sub 0.5}Pr{sub 0.5}FeO{sub 3} single crystal. The single crystal of about 6 mm in diameter and 50 mm in length was successfully grown by optical floating zone method. Both X-ray diffraction and Laue photograph confirmed the homogeneity and high quality of the crystal. Magnetic properties of Ho{sub 0.5}Pr{sub 0.5}FeO{sub 3} single crystal are studied over a wide temperature range from 2 to 300 K. Spin reorientation transition from Γ{sub 2} to Γ{sub 4} phase is observed in the temperature range of 75–90 K. At lower temperature, the Ho{sub 0.5}Pr{sub 0.5}FeO{sub 3} shows an abrupt jump of magnetization along the a-axis, which occurs only in the field-cooling process, and is sensitive to external applied magnetic field. By analyzing the jump temperature and magnitude of the magnetization, we conclude that it is caused by the spin reversal of the rare earth ions. The isothermal magnetization versus field hysteresis loop measurements along a axis explain the spin configuration variation from 3 K to 60 K. - Highlights: • Ho{sub 0.5}Pr{sub 0.5}FeO{sub 3} single crystal was grown by optical floating zone method. • It shows an abrupt jump of magnetization along a axis at low temperature. • The jump height and temperature is sensitive to external applied magnetic field. • It is attributed to the spin reversal of the rare earth ions.

Radiation self-polarization of electrons moving in a magnetic field. [Vector spin operator, relaxation time

Energy Technology Data Exchange (ETDEWEB)

Bagrov, V G; Dorofeev, O F; Sokolov, A A; Ternov, I M; Khalilov, V R [Moskovskij Gosudarstvennyj Univ. (USSR)

1975-03-11

When electrons move in a magnetic field, synchrotron radiation gives rise to transitions accompanied by the electron spin reorientation. In this case, it is essential that the transition probability depends on the spin orientation; as a result electron polarization takes place with the spin orientation being predominantly opposite to the direction of the magnetic field. This effect has been called ''radiative self-polarization of electrons''. The present work is concerned with the question how the choice of the spin operator will affect the self-polarization degree and relaxation time. The problem has been solved for a vector spin operator.

Quenching of spin-flip quadrupole transitions

International Nuclear Information System (INIS)

Castel, B.; Blunden, P.; Okuhara, Y.

1985-01-01

An increasing amount of experimental data indicates that spin-flip quadrupole transitions exhibit quenching effects similar to those reported earlier in (p,n) reactions involving l = 0 and l = 1 transitions. We present here two model calculations suggesting that the E2 spin-flip transitions are more affected than their M1 and M3 counterparts by the tensor and spin-orbit components of the nuclear force and should exhibit the largest quenching. We also review the experimental evidence corroborating our observations

Spin reorientation phenomena in (R{sub 1-x}R`{sub x}){sub 2}Co{sub 14}B (R = La, R` = Dy and Ho)

Energy Technology Data Exchange (ETDEWEB)

Myojin, T. [Takamatsu Nat. Coll. of Technol. (Japan); Ohno, T. [Tokushima Univ. (Japan). Faculty of Engineering; Mizuno, K. [Tokushima Univ. (Japan). Faculty of Integrated Arts and Sciences; Tsujimura, A. [Faculty of Engineering, Tokushima Bunri Univ., Kagawa Shido (Japan); Kojima, K. [Hiroshima Univ. (Japan). Faculty of Integrated Arts and Sciences

1997-07-01

The variations of magnetization with temperature in (La{sub 1-x}R`{sub x}){sub 2}Co{sub 14}B (R` = Dy and Ho) have been measured to determine spin reorientation temperature T{sub SR} of these compounds. The phase diagrams of spin arrangement thus obtained indicate monotonous increase in T{sub SR} with R` concentration x. Also, T{sub SR}`s of R{sub 2}Co{sub 14}B(R = Tb, Dy and Ho) are found to vary linearly with the Stevens factor {alpha} of R. (orig.). 4 refs.

Spin reorientation in (R[sub 1-x]R'[sub x])[sub 2]Co[sub 14]B (R=Y and Gd, R'=Tb, Dy and Ho). [YTbCoB; YDyCoB; YHoCoB; GdTbCoB; GdDyCoB; GdHoCoB

Energy Technology Data Exchange (ETDEWEB)

Myojin, T. (Takamatsu National Coll. of Technology, Takamatsu (Japan)); Ohno, T. (Faculty of Engineering, Tokushima Univ. (Japan)); Tsujimura, A. (Faculty of Engineering, Tokushima Bunri Univ., Kagawa Shido (Japan)); Hihara, T. (Faculty of Integrated Arts and Sciences, Hiroshima Univ. (Japan))

1994-02-01

In order to investigate spin reorientation mechanism microscopically, the constituent dependences of the spin reorientation temperature T[sub SR] have been determined in (R[sub 1-x]R'[sub x])[sub 2]Co[sub 14]B by magnetization and [sup 59]Co NMR measurements. The spin arrangement phase diagrams are prorosed and the results are discussed with the crystalline electric field effect and Co-R exchange interaction. (orig.)

Analysis of multi-step transitions in spin crossover nanochains

Energy Technology Data Exchange (ETDEWEB)

Chiruta, Daniel [GEMaC, Université de Versailles Saint-Quentin-en-Yvelines, CNRS-UVSQ (UMR 8635), 78035 Versailles Cedex (France); LISV, Université de Versailles Saint-Quentin-en-Yvelines, 78140 Velizy (France); Faculty of Electrical Engineering and Computer Science, Stefan cel Mare University, Suceava 720229 (Romania); Linares, Jorge, E-mail: jorge.linares@uvsq.fr [GEMaC, Université de Versailles Saint-Quentin-en-Yvelines, CNRS-UVSQ (UMR 8635), 78035 Versailles Cedex (France); Garcia, Yann, E-mail: yann.garcia@uclouvain.be [Institute of Condensed Matter and Nanosciences, Université Catholique de Louvain, Molecules, Solids and Reactivity (IMCN/MOST), Place Louis Pasteur, 1, 1348 Louvain-la-Neuve (Belgium); Dimian, Mihai [Faculty of Electrical Engineering and Computer Science, Stefan cel Mare University, Suceava 720229 (Romania); Dahoo, Pierre Richard [LATMOS, Université de Versailles-Saint-Quentin-en-Yvelines, CNRS-UPMC-UVSQ (UMR 8190), 78280 Guyancourt (France)

2014-02-01

The temperature driven phase transition occurring in spin crossover nanochains has been studied by an Ising-like model considering both short-range and long-range interactions. Various types of spin crossover profiles have been described in this framework, including a novel three-step transition identified in a nanosystem with eight molecules, which is modeled for the first time. A special interest has been also given to stepwise transitions accompanied by two hysteresis loops. The edge and size effects on spin crossover behavior have been investigated in order to get a deeper insight of the underlying mechanisms involved in these unusual spin transitions.

Spin-Orbitronics at Transition Metal Interfaces

KAUST Repository

Manchon, Aurelien

2017-11-09

The presence of large spin–orbit interaction at transition metal interfaces enables the emergence of a variety of fascinating phenomena that have been at the forefront of spintronics research in the past 10 years. The objective of the present chapter is to offer a review of these various effects from a theoretical perspective, with a particular focus on spin transport, chiral magnetism, and their interplay. After a brief description of the orbital hybridization scheme at transition metal interfaces, we address the impact of spin–orbit coupling on the interfacial magnetic configuration, through the celebrated Dzyaloshinskii–Moriya interaction. We then discuss the physics of spin transport and subsequent torques occurring at these interfaces. We particularly address the spin Hall, spin swapping, and inverse spin-galvanic effects. Finally, the interplay between flowing charges and chiral magnetic textures and their induced dynamics are presented. We conclude this chapter by proposing some perspectives on promising research directions.

Spin-Orbitronics at Transition Metal Interfaces

KAUST Repository

Manchon, Aurelien; Belabbes, Abderrezak

2017-01-01

The presence of large spin–orbit interaction at transition metal interfaces enables the emergence of a variety of fascinating phenomena that have been at the forefront of spintronics research in the past 10 years. The objective of the present chapter is to offer a review of these various effects from a theoretical perspective, with a particular focus on spin transport, chiral magnetism, and their interplay. After a brief description of the orbital hybridization scheme at transition metal interfaces, we address the impact of spin–orbit coupling on the interfacial magnetic configuration, through the celebrated Dzyaloshinskii–Moriya interaction. We then discuss the physics of spin transport and subsequent torques occurring at these interfaces. We particularly address the spin Hall, spin swapping, and inverse spin-galvanic effects. Finally, the interplay between flowing charges and chiral magnetic textures and their induced dynamics are presented. We conclude this chapter by proposing some perspectives on promising research directions.

Driving spin transition at interface: Role of adsorption configurations

Science.gov (United States)

Zhang, Yachao

2018-01-01

A clear insight into the electrical manipulation of molecular spins at interface is crucial to the design of molecule-based spintronic devices. Here we report on the electrically driven spin transition in manganocene physisorbed on a metallic surface in two different adsorption configurations predicted by ab initio techniques, including a Hubbard-U correction at the manganese site and accounting for the long-range van der Waals interactions. We show that the application of an electric field at the interface induces a high-spin to low-spin transition in the flat-lying manganocene, while it could hardly alter the high-spin ground state of the standing-up molecule. This phenomenon cannot be explained by either the molecule-metal charge transfer or the local electron correlation effects. We demonstrate a linear dependence of the intra-molecular spin-state splitting on the energy difference between crystal-field splitting and on-site Coulomb repulsion. After considering the molecule-surface binding energy shifts upon spin transition, we reproduce the obtained spin-state energetics. We find that the configuration-dependent responses of the spin-transition originate from the binding energy shifts instead of the variation of the local ligand field. Through these analyses, we obtain an intuitive understanding of the effects of molecule-surface contact on spin-crossover under electrical bias.

Spin-glass transition in disordered terbium

International Nuclear Information System (INIS)

Hauser, J.J.

1985-01-01

While crystalline Tb is a helix antiferromagnet with a Neel temperature of 229 K which becomes ferromagnetic at 222 K, disordered Tb exhibits a spin-glass transition. The spin-glass freezing temperature ranges from 183 to 53 K, the lowest temperatures corresponding to the greatest degree of atomic disorder. These experiments constitute the first evidence for an elemental spin-glass. (author)

Spin-orbit-induced spin splittings in polar transition metal dichalcogenide monolayers

KAUST Repository

Cheng, Yingchun; Zhu, Zhiyong; Tahir, Muhammad; Schwingenschlö gl, Udo

2013-01-01

. We present ab initio electronic structure, phonon, and molecular-dynamics calculations to study the structural stability and spin-orbit-induced spin splitting in the transition metal dichalcogenide monolayers MXY (M = Mo, W and X, Y = S, Se, Te

Spin-Hall effect and emergent antiferromagnetic phase transition in n-Si

Science.gov (United States)

Lou, Paul C.; Kumar, Sandeep

2018-04-01

Spin current experiences minimal dephasing and scattering in Si due to small spin-orbit coupling and spin-lattice interactions is the primary source of spin relaxation. We hypothesize that if the specimen dimension is of the same order as the spin diffusion length then spin polarization will lead to non-equilibrium spin accumulation and emergent phase transition. In n-Si, spin diffusion length has been reported up to 6 μm. The spin accumulation in Si will modify the thermal transport behavior of Si, which can be detected with thermal characterization. In this study, we report observation of spin-Hall effect and emergent antiferromagnetic phase transition behavior using magneto-electro-thermal transport characterization. The freestanding Pd (1 nm)/Ni80Fe20 (75 nm)/MgO (1 nm)/n-Si (2 μm) thin film specimen exhibits a magnetic field dependent thermal transport and spin-Hall magnetoresistance behavior attributed to Rashba effect. An emergent phase transition is discovered using self-heating 3ω method, which shows a diverging behavior at 270 K as a function of temperature similar to a second order phase transition. We propose that spin-Hall effect leads to the spin accumulation and resulting emergent antiferromagnetic phase transition. We propose that the length scale for Rashba effect can be equal to the spin diffusion length and two-dimensional electron gas is not essential for it. The emergent antiferromagnetic phase transition is attributed to the site inversion asymmetry in diamond cubic Si lattice.

Phase transitions and spin excitations of spin-1 bosons in optical lattice

Science.gov (United States)

Zhu, Min-Jie; Zhao, Bo

2018-03-01

For spin-1 bosonic system trapped in optical lattice, we investigate two main problems, including MI-SF phase transition and magnetic phase separations in MI phase, with extended standard basis operator (SBO) method. For both ferromagnetic (U2 0) systems, we analytically figure out the symmetry properties in Mott-insulator and superfluid phases, which would provide a deeper insight into the MI-SF phase transition process. Then by applying self-consistent approach to the method, we include the effect of quantum and thermal fluctuations and derive the MI-SF transition phase diagram, which is in quantitative agreement with recent Monte-Carlo simulation at zero temperature, and at finite temperature, we find the underestimation of finite-temperature-effect in the mean-field approximation method. If we further consider the spin excitations in the insulating states of spin-1 system in external field, distinct spin phases are expected. Therefore, in the Mott lobes with n = 1 and n = 2 atoms per site, we give analytical and numerical boundaries of the singlet, nematic, partially magnetic and ferromagnetic phases in the magnetic phase diagrams.

Spin transitions in semiconductor quantum rings

International Nuclear Information System (INIS)

Baxevanis, Benjamin; Pfannkuche, Daniela

2010-01-01

We adopt the path integral Monte Carlo method to accurately resolve the total spin of the ground state of electrons confined in a quantum ring with different geometries. Using this method, an evaluation of the ground state of three electrons in a ring shows a spin transition to the fully polarized state by increasing the radius and thereby enhancing the Coulomb interaction. The total spin of the ground state is determined by the mutual interplay of confinement and electron-electron interaction. An analysis of the four-electron ring demonstrates that in this case no spin transitions take place. Furthermore, the effect of geometric distortion of the ring on its ground state has been investigated. Elliptically deforming the ring breaks the symmetry of the system and leads to the removal of orbital degeneracy. For strong distortion the splitting between hybridized states is sufficient to overcome the exchange-energy saving associated with a higher spin state. We have found that this effect removes the polarization of three electrons. Even in a four-electron ring the ground state is forced by the distortion to be unpolarized and thus suppressing the Hund's rule ground state.

Revisiting the flocking transition using active spins.

Science.gov (United States)

Solon, A P; Tailleur, J

2013-08-16

We consider an active Ising model in which spins both diffuse and align on lattice in one and two dimensions. The diffusion is biased so that plus or minus spins hop preferably to the left or to the right, which generates a flocking transition at low temperature and high density. We construct a coarse-grained description of the model that predicts this transition to be a first-order liquid-gas transition in the temperature-density ensemble, with a critical density sent to infinity. In this first-order phase transition, the magnetization is proportional to the liquid fraction and thus varies continuously throughout the phase diagram. Using microscopic simulations, we show that this theoretical prediction holds in 2D whereas the fluctuations alter the transition in 1D, preventing, for instance, any spontaneous symmetry breaking.

Antiferromagnetic spin phase transition in nuclear matter with effective Gogny interaction

International Nuclear Information System (INIS)

Isayev, A.A.; Yang, J.

2004-01-01

The possibility of ferromagnetic and antiferromagnetic phase transitions in symmetric nuclear matter is analyzed within the framework of a Fermi liquid theory with the effective Gogny interaction. It is shown that at some critical density nuclear matter with the D1S effective force undergoes a phase transition to the antiferromagnetic spin state (opposite directions of neutron and proton spins). The self-consistent equations of spin polarized nuclear matter with the D1S force have no solutions corresponding to ferromagnetic spin ordering (the same direction of neutron and proton spins) and, hence, the ferromagnetic transition does not appear. The dependence of the antiferromagnetic spin polarization parameter as a function of density is found at zero temperature

Reorientation of magnetization with temperature in 2D ferromagnets

International Nuclear Information System (INIS)

Fridman, Yu. A.; Spirin, D.V.; Klevets, Ph. N.

2002-01-01

We investigated 2D Heisenberg ferromagnet (monolayer) with the account of dipolar forces and uniaxial anisotropy and found a reorientation phase transition in temperature from out-of-plane to in-plane phase. This phase transition is of the first order with hysteresis. We estimated the temperatures of switching both analytically and numerically

Spontaneous and field-induced phase transitions in TbFe.sub.5./sub.Al.sub.7./sub..

Czech Academy of Sciences Publication Activity Database

Gorbunov, Denis; Yasin, S.; Andreev, Alexander V.; Mushnikov, N. V.; Skourski, Y.; Zherlitsyn, S.; Wosnitza, J.

2014-01-01

Roč. 535, Sep (2014), 56-63 ISSN 0304-8853 R&D Projects: GA ČR GAP204/12/0150 Grant - others:AVČR(CZ) M100101203 Institutional support: RVO:68378271 Keywords : rare-earth intermetallics * ferrimagnetism * magnetic anisotropy * spin-reorientation transition * high magnetic fields * field-induced transition Subject RIV: BM - Solid Matter Physics ; Magnetism Impact factor: 1.970, year: 2014

Condensate-induced transitions and critical spin chains

NARCIS (Netherlands)

Månsson, T.; Lahtinen, V.; Suorsa, J.; Ardonne, E.

2013-01-01

We show that condensate-induced transitions between two-dimensional topological phases provide a general framework to relate one-dimensional spin models at their critical points. We demonstrate this using two examples. First, we show that two well-known spin chains, namely, the XY chain and the

Power-controlled transition from standard to negative refraction in reorientational soft matter.

Science.gov (United States)

Piccardi, Armando; Alberucci, Alessandro; Kravets, Nina; Buchnev, Oleksandr; Assanto, Gaetano

2014-11-25

Refraction at a dielectric interface can take an anomalous character in anisotropic crystals, when light is negatively refracted with incident and refracted beams emerging on the same side of the interface normal. In soft matter subject to reorientation, such as nematic liquid crystals, the nonlinear interaction with light allows tuning of the optical properties. We demonstrate that in such material a beam of light can experience either positive or negative refraction depending on input power, as it can alter the spatial distribution of the optic axis and, in turn, the direction of the energy flow when traveling across an interface. Moreover, the nonlinear optical response yields beam self-focusing and spatial localization into a self-confined solitary wave through the formation of a graded-index waveguide, linking the refractive transition to power-driven readdressing of copolarized guided-wave signals, with a number of output ports not limited by diffraction.

Oxidation-induced spin reorientation in Co adatoms and CoPd dimers on Ni/Cu(100)

Science.gov (United States)

Chen, K.; Beeck, T.; Fiedler, S.; Baev, I.; Wurth, W.; Martins, M.

2016-04-01

Ultrasmall magnetic clusters and adatoms are of strong current interest because of their possible use in future technological applications. Here, we demonstrate that the magnetic coupling between the adsorbates and the substrate can be significantly changed through oxidation. The magnetic properties of Co adatoms and CoPd dimers deposited on a remanently magnetized Ni/Cu(100) substrate have been investigated by x-ray absorption and x-ray magnetic circular dichroism spectroscopy at the Co L2 ,3 edges. Using spectral differences, pure and oxidized components are distinguished, and their respective magnetic moments are determined. The Co adatoms and the CoPd dimers are coupled ferromagnetically to the substrate, while their oxides, Co-O and CoPd-O, are coupled antiferromagnetically to the substrate. Along with the spin reorientation from the pure to the oxidized state, the magnetic moment of the adatom is highly reduced from Co to Co-O. In contrast, the magnetic moment of the dimer is of similar order for CoPd and CoPd-O.

Phase transitions of anisotropic and exchange origins in TmFe.sub.5./sub.Al.sub.7./sub

Czech Academy of Sciences Publication Activity Database

Gorbunov, Denis; Yasin, S.; Andreev, Alexander V.; Mushnikov, N. V.; Rosenfeld, E.V.; Skourski, Y.; Zherlitsyn, S.; Wosnitza, J.

2014-01-01

Roč. 89, č. 21 (2014), "214417-1"-"214417-9" ISSN 1098-0121 R&D Projects: GA ČR GAP204/12/0150 Grant - others:AVČR(CZ) M100101203 Institutional support: RVO:68378271 Keywords : rare-earth intermetallics * ferrimagnetism * magnetic anisotropy * spin-reorientation transition * high magnetic fields * field-induced transition Subject RIV: BM - Solid Matter Physics ; Magnetism Impact factor: 3.736, year: 2014

Tunable spin-charge conversion through topological phase transitions in zigzag nanoribbons

KAUST Repository

Li, Hang

2016-06-29

We study spin-orbit torques and charge pumping in magnetic quasi-one-dimensional zigzag nanoribbons with a hexagonal lattice, in the presence of large intrinsic spin-orbit coupling. Such a system experiences a topological phase transition from a trivial band insulator to a quantum spin Hall insulator by tuning of either the magnetization direction or the intrinsic spin-orbit coupling. We find that the spin-charge conversion efficiency (i.e., spin-orbit torque and charge pumping) is dramatically enhanced at the topological transition, displaying a substantial angular anisotropy.

Tunable spin-charge conversion through topological phase transitions in zigzag nanoribbons

KAUST Repository

Li, Hang; Manchon, Aurelien

2016-01-01

We study spin-orbit torques and charge pumping in magnetic quasi-one-dimensional zigzag nanoribbons with a hexagonal lattice, in the presence of large intrinsic spin-orbit coupling. Such a system experiences a topological phase transition from a trivial band insulator to a quantum spin Hall insulator by tuning of either the magnetization direction or the intrinsic spin-orbit coupling. We find that the spin-charge conversion efficiency (i.e., spin-orbit torque and charge pumping) is dramatically enhanced at the topological transition, displaying a substantial angular anisotropy.

Giant spin-orbit-induced spin splitting in two-dimensional transition-metal dichalcogenide semiconductors

KAUST Repository

Zhu, Zhiyong

2011-10-14

Fully relativistic first-principles calculations based on density functional theory are performed to study the spin-orbit-induced spin splitting in monolayer systems of the transition-metal dichalcogenides MoS2, MoSe2, WS2, and WSe2. All these systems are identified as direct-band-gap semiconductors. Giant spin splittings of 148–456 meV result from missing inversion symmetry. Full out-of-plane spin polarization is due to the two-dimensional nature of the electron motion and the potential gradient asymmetry. By suppression of the Dyakonov-Perel spin relaxation, spin lifetimes are expected to be very long. Because of the giant spin splittings, the studied materials have great potential in spintronics applications.

Giant spin-orbit-induced spin splitting in two-dimensional transition-metal dichalcogenide semiconductors

KAUST Repository

Zhu, Zhiyong; Cheng, Yingchun; Schwingenschlö gl, Udo

2011-01-01

Fully relativistic first-principles calculations based on density functional theory are performed to study the spin-orbit-induced spin splitting in monolayer systems of the transition-metal dichalcogenides MoS2, MoSe2, WS2, and WSe2. All these systems are identified as direct-band-gap semiconductors. Giant spin splittings of 148–456 meV result from missing inversion symmetry. Full out-of-plane spin polarization is due to the two-dimensional nature of the electron motion and the potential gradient asymmetry. By suppression of the Dyakonov-Perel spin relaxation, spin lifetimes are expected to be very long. Because of the giant spin splittings, the studied materials have great potential in spintronics applications.

Quantum phase transitions in random XY spin chains

International Nuclear Information System (INIS)

Bunder, J.E.; McKenzie, R.H.

2000-01-01

Full text: The XY spin chain in a transverse field is one of the simplest quantum spin models. It is a reasonable model for heavy fermion materials such as CeCu 6-x Au x . It has two quantum phase transitions: the Ising transition and the anisotropic transition. Quantum phase transitions occur at zero temperature. We are investigating what effect the introduction of randomness has on these quantum phase transitions. Disordered systems which undergo quantum phase transitions can exhibit new universality classes. The universality class of a phase transition is defined by the set of critical exponents. In a random system with quantum phase transitions we can observe Griffiths-McCoy singularities. Such singularities are observed in regions which have no long range order, so they are not classified as critical regions, yet they display phenomena normally associated with critical points, such as a diverging susceptibility. Griffiths-McCoy phases are due to rare regions with stronger than! average interactions and may be present far from the quantum critical point. We show how the random XY spin chain may be mapped onto a random Dirac equation. This allows us to calculate the density of states without making any approximations. From the density of states we can describe the conditions which should allow a Griffiths-McCoy phase. We find that for the Ising transition the dynamic critical exponent, z, is not universal. It is proportional to the disorder strength and inversely proportional to the energy gap, hence z becomes infinite at the critical point where the energy gap vanishes

Sudden transition and sudden change from open spin environments

International Nuclear Information System (INIS)

Hu, Zheng-Da; Xu, Jing-Bo; Yao, Dao-Xin

2014-01-01

We investigate the necessary conditions for the existence of sudden transition or sudden change phenomenon for appropriate initial states under dephasing. As illustrative examples, we study the behaviors of quantum correlation dynamics of two noninteracting qubits in independent and common open spin environments, respectively. For the independent environments case, we find that the quantum correlation dynamics is closely related to the Loschmidt echo and the dynamics exhibits a sudden transition from classical to quantum correlation decay. It is also shown that the sudden change phenomenon may occur for the common environment case and stationary quantum discord is found at the high temperature region of the environment. Finally, we investigate the quantum criticality of the open spin environment by exploring the probability distribution of the Loschmidt echo and the scaling transformation behavior of quantum discord, respectively. - Highlights: • Sudden transition or sudden change from open spin baths are studied. • Quantum discord is related to the Loschmidt echo in independent open spin baths. • Steady quantum discord is found in a common open spin bath. • The probability distribution of the Loschmidt echo is analyzed. • The scaling transformation behavior of quantum discord is displayed

Quantum spin-glass transition in the two-dimensional electron gas

Indian Academy of Sciences (India)

Home; Journals; Pramana – Journal of Physics; Volume 58; Issue 2 ... Spin glasses; quantum phase transition; ferromagnetism; electron gas. ... We argue that a quantum transition involving the destruction of the spin-glass order in an applied in-plane magnetic field offers a natural explanation of some features of recent ...

Theory of phase transformation and reorientation in single crystalline shape memory alloys

International Nuclear Information System (INIS)

Zhu, J J; Liang, N G; Cai, M; Liew, K M; Huang, W M

2008-01-01

A constitutive model, based on an (n+1)-phase mixture of the Mori–Tanaka average theory, has been developed for stress-induced martensitic transformation and reorientation in single crystalline shape memory alloys. Volume fractions of different martensite lattice correspondence variants are chosen as internal variables to describe microstructural evolution. Macroscopic Gibbs free energy for the phase transformation is derived with thermodynamics principles and the ensemble average method of micro-mechanics. The critical condition and the evolution equation are proposed for both the phase transition and reorientation. This model can also simulate interior hysteresis loops during loading/unloading by switching the critical driving forces when an opposite transition takes place

Continuous reorientation of synchronous terrestrial planets due to mantle convection

Science.gov (United States)

Leconte, Jérémy

2018-02-01

Many known rocky exoplanets are thought to have been spun down by tidal interactions to a state of synchronous rotation, in which a planet's period of rotation is equal to that of its orbit around its host star. Investigations into atmospheric and surface processes occurring on such exoplanets thus commonly assume that day and night sides are fixed with respect to the surface over geological timescales. Here we use an analytical model to show that true polar wander—where a planetary body's spin axis shifts relative to its surface because of changes in mass distribution—can continuously reorient a synchronous rocky exoplanet. As occurs on Earth, we find that even weak mantle convection in a rocky exoplanet can produce density heterogeneities within the mantle sufficient to reorient the planet. Moreover, we show that this reorientation is made very efficient by the slower rotation rate of a synchronous planet when compared with Earth, which limits the stabilizing effect of rotational and tidal deformations. Furthermore, a relatively weak lithosphere limits its ability to support remnant loads and stabilize against reorientation. Although uncertainties exist regarding the mantle and lithospheric evolution of these worlds, we suggest that the axes of smallest and largest moment of inertia of synchronous exoplanets with active mantle convection change continuously over time, but remain closely aligned with the star-planet and orbital axes, respectively.

Behavior learning in differential games and reorientation maneuvers

Science.gov (United States)

Satak, Neha

method is the Direct Approximation of Value Function (DAVF) method. In this method, unlike the CSR method, the player formulates an objective function for the opponent but does not formulates a strategy directly; rather, indirectly the player assumes that the opponent is playing optimally. Thus, a value function satisfying the HJB equation corresponding to the opponent's cost function exists. The DAVF method finds an approximate solution for the value function based on previous observations of the opponent's control. The approximate solution to the value function is then used to predict the opponent's future behavior. Game examples in which only a single player is learning its opponent's behavior are simulated. Subsequently, examples in which both players in a two-player game are learning each other's behavior are simulated. In the second part of this research, a reorientation control maneuver for a spinning spacecraft will be developed. This will aid the application of behavior learning and differential games concepts to the specific scenario involving multiple spinning spacecraft. An impulsive reorientation maneuver with coasting will be analytically designed to reorient the spin axis of the spacecraft using a single body fixed thruster. Cooperative maneuvers of multiple spacecraft optimizing fuel and relative orientation will be designed. Pareto optimality concepts will be used to arrive at mutually agreeable reorientation maneuvers for the cooperating spinning spacecraft.

Spin Properties of Transition-Metallorganic Self-Assembled Molecules

International Nuclear Information System (INIS)

Yu, Zhi Gang

2010-01-01

This report summarizes SRI's accomplishments on the project, 'Spin Properties of Transition-Metallorganic Self-Assembled Molecules' funded by the Office of Basic Energy Sciences, US Department of Energy. We have successfully carried out all tasks identified in our proposal and gained significant knowledge and understanding of spin-polarized electronic structure, spin relaxation, and spin-dependent transport in transition-metallorganic molecules and enhohedral fullerenes. These molecules contain integrated spin and charge components and will enable us to achieve sophisticated functions in spintronics and quantum computing at molecular level with simple circuitry and easy fabrication. We have developed microscopic theories that describe the underlying mechanisms of spin-dependent porcesses and constructed quantitative modeling tools that compute several important spin properties. These results represent the basic principles governing the spin-dependent behaviors in nanostructures containing such molecules. Based on these results we have shown that novel device functions, such as electrically controlled g-factor and noninvasive electrical detection of spin dynamics, can be achieved in these nanostructures. Some of our results have been published in peer-reviewed journals and presented at professional conferences. In addition, we have established a close collaboration with experimentalists at Oxford University, UK (Dr. J. Morton and Prof. G. Briggs), Princeton University (Dr. A. Tyryshkin and Prof. S. Lyon), University of Delaware (Prof. E. Nowak), and University of California (Profs. R. Kawakami and J. Shi), who have been studying related systems and supplying us with new experimental data. We have provided our understanding and physical insights to the experimentalists and helped analyze their experimental measurements. The collaboration with experimentalists has also broadened our research scope and helped us focus on the most relevant issues concerning these

Spin rotation in ErGa{sub 3}

Energy Technology Data Exchange (ETDEWEB)

Murasik, A. E-mail: amur@cyf.gov.pl; Czopnik, A. E-mail: czopnik@int.pan.wroc.pl; Keller, L. E-mail: lukas.keller@psi.ch; Fischer, P. E-mail: peter.fischer@psi.ch

2000-04-01

The magnetic phase diagram of ErGa{sub 3}, built up from bulk magnetisation data, shows in zero-applied magnetic field two successive transitions at T{sub 1}=2.6 and T{sub 2} congruent with 2.8 K, respectively. The magnetic ordering of ErGa{sub 3} examined by neutron diffraction, can be derived from the so-called {l_brace}((1)/(2)), ((1)/(2)), 0{r_brace} structure, i.e. one in which the successive antiparallel (1 1 0) sheets of spins have additionally superimposed on them a sinusoidal modulation parallel to the [1 0 0] axis. The temperature dependence of neutron diffraction diagrams studied on the single crystal, revealed in the range of (2.6-2.78) K an abrupt reorientation of the Er{sup 3+} spins from the nearly [1 1 0] direction, towards the [1 0 0] axis. In this way previously observed effect on the polycrystalline sample has been confirmed. This rotation can be attributed to the T{sub 1} transition found in the H-T magnetic phase diagram.

Spin-flip transitions between Zeeman sublevels in semiconductor quantum dots

International Nuclear Information System (INIS)

Khaetskii, Alexander V.; Nazarov, Yuli V.

2001-01-01

We have studied spin-flip transitions between Zeeman sublevels in GaAs electron quantum dots. Several different mechanisms which originate from spin-orbit coupling are shown to be responsible for such processes. It is shown that spin-lattice relaxation for the electron localized in a quantum dot is much less effective than for the free electron. The spin-flip rates due to several other mechanisms not related to the spin-orbit interaction are also estimated

Nanopolar reorientation in ferroelectric thin films

International Nuclear Information System (INIS)

Hubert, C.; Levy, J.; Rivkin, T. V.; Carlson, C.; Parilla, P. A.; Perkins, J. D.; Ginley, D. S.

2001-01-01

The influence of varying oxygen pressure P(O 2 ) during the growth of Ba 0.4 Sr 0.6 TiO 3 thin films is investigated using dielectric and local optical probes. A transition from in-plane to out-of-plane ferroelectricity is observed with increasing P(O 2 ). Signatures of in-plane and out-of-plane ferroelectricity are identified using dielectric response and time-resolved confocal scanning optical microscopy (TRCSOM). At the crossover pressure between in-plane and out-of-plane polarization (P c =85 mTorr), TRCSOM measurements reveal a soft, highly dispersive out-of-plane polarization that reorients in plane under modest applied electric fields. At higher deposition pressures, the out-of-plane polarization is hardened and is less dispersive at microwave frequencies, and the dielectric tuning is suppressed. Nanopolar reorientation is believed to be responsible for the marked increase in dielectric tuning at P(O 2 )=P c

Spin Properties of Transition-Metallorganic Self-Assembled Molecules

Energy Technology Data Exchange (ETDEWEB)

Zhi Gang Yu

2010-06-30

This report summarizes SRI's accomplishments on the project, 'Spin Properties of Transition-Metallorganic Self-Assembled Molecules' funded by the Office of Basic Energy Sciences, US Department of Energy. We have successfully carried out all tasks identified in our proposal and gained significant knowledge and understanding of spin-polarized electronic structure, spin relaxation, and spin-dependent transport in transition-metallorganic molecules and enhohedral fullerenes. These molecules contain integrated spin and charge components and will enable us to achieve sophisticated functions in spintronics and quantum computing at molecular level with simple circuitry and easy fabrication. We have developed microscopic theories that describe the underlying mechanisms of spin-dependent porcesses and constructed quantitative modeling tools that compute several important spin properties. These results represent the basic principles governing the spin-dependent behaviors in nanostructures containing such molecules. Based on these results we have shown that novel device functions, such as electrically controlled g-factor and noninvasive electrical detection of spin dynamics, can be achieved in these nanostructures. Some of our results have been published in peer-reviewed journals and presented at professional conferences. In addition, we have established a close collaboration with experimentalists at Oxford University, UK (Dr. J. Morton and Prof. G. Briggs), Princeton University (Dr. A. Tyryshkin and Prof. S. Lyon), University of Delaware (Prof. E. Nowak), and University of California (Profs. R. Kawakami and J. Shi), who have been studying related systems and supplying us with new experimental data. We have provided our understanding and physical insights to the experimentalists and helped analyze their experimental measurements. The collaboration with experimentalists has also broadened our research scope and helped us focus on the most relevant issues

Role of entropy and structural parameters in the spin-state transition of LaCoO3

Science.gov (United States)

Chakrabarti, Bismayan; Birol, Turan; Haule, Kristjan

2017-11-01

The spin-state transition in LaCoO3 has eluded description for decades despite concerted theoretical and experimental effort. In this study, we approach this problem using fully charge self-consistent density functional theory + embedded dynamical mean field theory (DFT+DMFT). We show from first principles that LaCoO3 cannot be described by a single, pure spin state at any temperature. Instead, we observe a gradual change in the population of higher-spin multiplets with increasing temperature, with the high-spin multiplets being excited at the onset of the spin-state transition followed by the intermediate-spin multiplets being excited at the metal-insulator-transition temperature. We explicitly elucidate the critical role of lattice expansion and oxygen octahedral rotations in the spin-state transition. We also reproduce, from first principles, that the spin-state transition and the metal-insulator transition in LaCoO3 occur at different temperature scales. In addition, our results shed light on the importance of electronic entropy in driving the spin-state transition, which has so far been ignored in all first-principles studies of this material.

Spin-orbit-induced spin splittings in polar transition metal dichalcogenide monolayers

KAUST Repository

Cheng, Yingchun

2013-06-01

The Rashba effect in quasi two-dimensional materials, such as noble metal surfaces and semiconductor heterostructures, has been investigated extensively, while interest in real two-dimensional systems has just emerged with the discovery of graphene. We present ab initio electronic structure, phonon, and molecular-dynamics calculations to study the structural stability and spin-orbit-induced spin splitting in the transition metal dichalcogenide monolayers MXY (M = Mo, W and X, Y = S, Se, Te). In contrast to the non-polar systems with X = Y, in the polar systems with X ≠ Y the Rashba splitting at the Γ-point for the uppermost valence band is caused by the broken mirror symmetry. An enhancement of the splitting can be achieved by increasing the spin-orbit coupling and/or the potential gradient. © Copyright EPLA, 2013.

Spatiotemporal dynamics of the spin transition in [Fe (HB(tz)3) 2] single crystals

Science.gov (United States)

Ridier, Karl; Rat, Sylvain; Shepherd, Helena J.; Salmon, Lionel; Nicolazzi, William; Molnár, Gábor; Bousseksou, Azzedine

2017-10-01

The spatiotemporal dynamics of the spin transition have been thoroughly investigated in single crystals of the mononuclear spin-crossover (SCO) complex [Fe (HB (tz )3)2] (tz = 1 ,2 ,4-triazol-1-yl) by optical microscopy. This compound exhibits an abrupt spin transition centered at 334 K with a narrow thermal hysteresis loop of ˜1 K (first-order transition). Most single crystals of this compound reveal exceptional resilience upon repeated switching (several hundred cycles), which allowed repeatable and quantitative measurements of the spatiotemporal dynamics of the nucleation and growth processes to be carried out. These experiments revealed remarkable properties of the thermally induced spin transition: high stability of the thermal hysteresis loop, unprecedented large velocities of the macroscopic low-spin/high-spin phase boundaries up to 500 µm/s, and no visible dependency on the temperature scan rate. We have also studied the dynamics of the low-spin → high-spin transition induced by a local photothermal excitation generated by a spatially localized (Ø = 2 μ m ) continuous laser beam. Interesting phenomena have been evidenced both in quasistatic and dynamic conditions (e.g., threshold effects and long incubation periods, thermal activation of the phase boundary propagation, stabilization of the crystal in a stationary biphasic state, and thermal cutoff frequency). These measurements demonstrated the importance of thermal effects in the transition dynamics, and they enabled an accurate determination of the thermal properties of the SCO compound in the framework of a simple theoretical model.

Quantum Phase Transition in a Cold Atomic Spin-Boson Mixture

Science.gov (United States)

Orth, Peter P.; Stanic, Ivan; Le Hur, Karyn

2008-03-01

We theoretically implement a spin array in a tunable bosonic environment using cold bosonic atoms with two (hyperfine) ground states, trapped by different potentials [1]. The first specie lies in a deep optical lattice with tightly confining wells and forms a spin array; spin-up/down corresponds to occupation by one/no atom at each site. The second specie forms a superfluid reservoir. Different species are coupled coherently via laser transitions and collisions. Whereas the laser coupling mimics a transverse field for the spins, the coupling to the reservoir phonons (sound modes) induces a ferromagnetic (Ising) coupling as well as dissipation. This results in a peculiar ferro-paramagnetic quantum phase transition where the effect of dissipation can be studied in a controllable manner. [1] Peter P. Orth, Ivan Stanic, and Karyn Le Hur, arXiv:0711.2309 [cond-mat.other].

Spin Structures in Magnetic Nanoparticles

DEFF Research Database (Denmark)

Mørup, Steen; Brok, Erik; Frandsen, Cathrine

2013-01-01

Spin structures in nanoparticles of ferrimagnetic materials may deviate locally in a nontrivial way from ideal collinear spin structures. For instance, magnetic frustration due to the reduced numbers of magnetic neighbors at the particle surface or around defects in the interior can lead to spin...... canting and hence a reduced magnetization. Moreover, relaxation between almost degenerate canted spin states can lead to anomalous temperature dependences of the magnetization at low temperatures. In ensembles of nanoparticles, interparticle exchange interactions can also result in spin reorientation....... Here, we give a short review of anomalous spin structures in nanoparticles....

Driven spin transitions in fluorinated single- and bilayer-graphene quantum dots

Science.gov (United States)

Żebrowski, D. P.; Peeters, F. M.; Szafran, B.

2017-06-01

Spin transitions driven by a periodically varying electric potential in dilute fluorinated graphene quantum dots are investigated. Flakes of monolayer graphene as well as electrostatic electron traps induced in bilayer graphene are considered. The stationary states obtained within the tight-binding approach are used as the basis for description of the system dynamics. The dilute fluorination of the top layer lifts the valley degeneracy of the confined states and attenuates the orbital magnetic dipole moments due to current circulation within the flake. The spin-orbit coupling introduced by the surface deformation of the top layer induced by the adatoms allows the spin flips to be driven by the AC electric field. For the bilayer quantum dots the spin flip times is substantially shorter than the spin relaxation. Dynamical effects including many-photon and multilevel transitions are also discussed.

Hydrostatic-pressure and uniaxial-strain experiments for controlling the spin-Peierls transition

International Nuclear Information System (INIS)

Mito, Masaki; Deguchi, Hiroyuki; Fujita, Wataru; Kondo, Ryusuke; Kagoshima, Seiichi

2010-01-01

The spin-Peierls (SP) system is considered to be a quantum spin system strongly coupled with the lattice. We have succeeded in controlling SP transition by applying hydrostatic pressure and/or uniaxial strain. The observed phenomenon could be a typical example for understanding the SP transition based on the Hamiltonian. (author)

Electron spin relaxation in a transition-metal dichalcogenide quantum dot

Science.gov (United States)

Pearce, Alexander J.; Burkard, Guido

2017-06-01

We study the relaxation of a single electron spin in a circular quantum dot in a transition-metal dichalcogenide monolayer defined by electrostatic gating. Transition-metal dichalcogenides provide an interesting and promising arena for quantum dot nano-structures due to the combination of a band gap, spin-valley physics and strong spin-orbit coupling. First we will discuss which bound state solutions in different B-field regimes can be used as the basis for qubits states. We find that at low B-fields combined spin-valley Kramers qubits to be suitable, while at large magnetic fields pure spin or valley qubits can be envisioned. Then we present a discussion of the relaxation of a single electron spin mediated by electron-phonon interaction via various different relaxation channels. In the low B-field regime we consider the spin-valley Kramers qubits and include impurity mediated valley mixing which will arise in disordered quantum dots. Rashba spin-orbit admixture mechanisms allow for relaxation by in-plane phonons either via the deformation potential or by piezoelectric coupling, additionally direct spin-phonon mechanisms involving out-of-plane phonons give rise to relaxation. We find that the relaxation rates scale as \\propto B 6 for both in-plane phonons coupling via deformation potential and the piezoelectric effect, while relaxation due to the direct spin-phonon coupling scales independant to B-field to lowest order but depends strongly on device mechanical tension. We will also discuss the relaxation mechanisms for pure spin or valley qubits formed in the large B-field regime.

Influence of longitudinal spin fluctuations on the phase transition features in chiral magnets

Science.gov (United States)

Belemuk, A. M.; Stishov, S. M.

2018-04-01

Using the classical Monte Carlo calculations, we investigate the effects of longitudinal spin fluctuations on the helimagnetic transition in a Heisenberg magnet with the Dzyaloshinskii-Moriya interaction. We use variable spin amplitudes in the framework of the spin-lattice Hamiltonian. It is this kind of fluctuations that naturally occur in an itinerant system. We show that the basic features of the helical phase transition are not changed much by the longitudinal spin fluctuations though the transition temperature Tc and the fluctuation hump seen in specific heat at T >Tc is significantly affected. We report thermodynamic and structural effects of these fluctuations. By increasing the system size in the Monte Carlo modeling, we are able to reproduce the ring shape scattering intensity above the helimagnetic transition temperature Tc, which transforms into the spiral spots seen below Tc in the neutron scattering experiments.

Electron spin transition causing structure transformations of earth's interiors under high pressure

Science.gov (United States)

Yamanaka, T.; Kyono, A.; Kharlamova, S.; Alp, E.; Bi, W.; Mao, H.

2012-12-01

To elucidate the correlation between structure transitions and spin state is one of the crucial problems for understanding the geophysical properties of earth interiors under high pressure. High-pressure studies of iron bearing spinels attract extensive attention in order to understand strong electronic correlation such as the charge transfer, electron hopping, electron high-low spin transition, Jahn-Teller distortion and charge disproponation in the lower mantle or subduction zone [1]. Experiment Structure transitions of Fe3-xSixO4, Fe3-xTixO4 Fe3-xCrxO4 spinel solid solution have been investigated at high pressure up to 60 GPa by single crystal and powder diffraction studies using synchrotron radiation with diamond anvil cell. X-ray emission experiment (XES) at high pressure proved the spin transition of Fe-Kβ from high spin (HS) to intermediate spin state (IS) or low spin state (LS). Mössbauer experiment and Raman spectra study have been also conducted for deformation analysis of Fe site and confirmation of the configuration change of Fe atoms. Jahn-Teller effect A cubic-to-tetragonal transition under pressure was induced by Jahn-Teller effect of IVFe2+ (3d6) in the tetrahedral site of Fe2TiO4 and FeCr2O4, providing the transformation from 43m (Td) to 42m (D2d). Tetragonal phase is formed by the degeneracy of e orbital of Fe2+ ion. Their c/a ratios are c/adisordered in the M2 site. At pressures above 53 GPa, Fe2TiO4 structure further transforms to Pmma. This structure change results in the order-disorder transition [2]. New structure of Fe2SiO4 The spin transition exerts an influence to Fe2SiO4 spinel structure and triggers two distinct curves of the lattice constant in the spinel phase. The reversible structure transition from cubic to pseudo-rhombohedral phase was observed at about 45 GPa. This transition is induced by the 20% shrinkage of ionic radius of VIFe2+at the low sin state. Laser heating experiment at 1500 K has confirmed the decomposition from the

Chiral-glass transition and replica symmetry breaking of a three-dimensional Heisenberg spin glass

OpenAIRE

Hukushima, K.; Kawamura, H.

2000-01-01

Extensive equilibrium Monte Carlo simulations are performed for a three-dimensional Heisenberg spin glass with the nearest-neighbor Gaussian coupling to investigate its spin-glass and chiral-glass orderings. The occurrence of a finite-temperature chiral-glass transition without the conventional spin-glass order is established. Critical exponents characterizing the transition are different from those of the standard Ising spin glass. The calculated overlap distribution suggests the appearance ...

Spherical 2+p spin-glass model: An exactly solvable model for glass to spin-glass transition

International Nuclear Information System (INIS)

Crisanti, A.; Leuzzi, L.

2004-01-01

We present the full phase diagram of the spherical 2+p spin-glass model with p≥4. The main outcome is the presence of a phase with both properties of full replica symmetry breaking phases of discrete models, e.g., the Sherrington-Kirkpatrick model, and those of one replica symmetry breaking. This phase has a finite complexity which leads to different dynamic and static properties. The phase diagram is rich enough to allow the study of different kinds of glass to spin glass and spin glass to spin glass phase transitions

Spin-flip transition of L10-type MnPt alloy single crystal studied by neutron scattering

International Nuclear Information System (INIS)

Hama, Hiroaki; Motomura, Ryo; Shinozaki, Tatsuya; Tsunoda, Yorihiko

2007-01-01

Magnetic structure, tetragonality, and the spin-flip transition for an L1 0 -type MnPt ordered alloy were studied by neutron scattering using a single-crystal specimen. Tetragonality of the lattice showed strong correlation with the spin-flip transition. Although the spin-flip transition looks like a gradual change of the easy axis in the temperature range between 580 and 770 K, two modes of magnon-gap peaks with different energies were observed in this transition temperature range. Thus, the crystal consists of two regions with different anisotropy energies and the volume fractions of these regions with different spin directions change gradually with temperature. The tetragonality and spin-flip transition are discussed using the hard-sphere model for atomic radii of Pt and Mn. The Invar effect of Mn atoms is proposed using high- and low-spin transitions of Mn moments in analogy with the two-γ model of Fe moments in FeNi Invar alloy

High-frequency EPR on high-spin transition-metal sites

NARCIS (Netherlands)

Mathies, Guinevere

2012-01-01

The electronic structure of transition-metal sites can be probed by electron-paramagnetic-resonance (EPR) spectroscopy. The study of high-spin transition-metal sites benefits from EPR spectroscopy at frequencies higher than the standard 9.5 GHz. However, high-frequency EPR is a developing field. In

Topological phase transition in anisotropic square-octagon lattice with spin-orbit coupling and exchange field

Science.gov (United States)

Yang, Yuan; Yang, Jian; Li, Xiaobing; Zhao, Yue

2018-03-01

We investigate the topological phase transitions in an anisotropic square-octagon lattice in the presence of spin-orbit coupling and exchange field. On the basis of the Chern number and spin Chern number, we find a number of topologically distinct phases with tuning the exchange field, including time-reversal-symmetry-broken quantum spin Hall phases, quantum anomalous Hall phases and a topologically trivial phase. Particularly, we observe a coexistent state of both the quantum spin Hall effect and quantum anomalous Hall effect. Besides, by adjusting the exchange filed, we find the phase transition from time-reversal-symmetry-broken quantum spin Hall phase to spin-imbalanced and spin-polarized quantum anomalous Hall phases, providing an opportunity for quantum spin manipulation. The bulk band gap closes when topological phase transitions occur between different topological phases. Furthermore, the energy and spin spectra of the edge states corresponding to different topological phases are consistent with the topological characterization based on the Chern and spin Chern numbers.

Dissipation-driven quantum phase transitions in collective spin systems

International Nuclear Information System (INIS)

Morrison, S; Parkins, A S

2008-01-01

We consider two different collective spin systems subjected to strong dissipation-on the same scale as interaction strengths and external fields-and show that either continuous or discontinuous dissipative quantum phase transitions can occur as the dissipation strength is varied. First, we consider a well-known model of cooperative resonance fluorescence that can exhibit a second-order quantum phase transition, and analyse the entanglement properties near the critical point. Next, we examine a dissipative version of the Lipkin-Meshkov-Glick interacting collective spin model, where we find that either first- or second-order quantum phase transitions can occur, depending only on the ratio of the interaction and external field parameters. We give detailed results and interpretation for the steady-state entanglement in the vicinity of the critical point, where it reaches a maximum. For the first-order transition we find that the semiclassical steady states exhibit a region of bistability. (fast track communication)

Spin-Driven Emergent Antiferromagnetism and Metal-Insulator Transition in Nanoscale p-Si

Science.gov (United States)

Lou, Paul C.; Kumar, Sandeep

2018-04-01

The entanglement of the charge, spin and orbital degrees of freedom can give rise to emergent behavior especially in thin films, surfaces and interfaces. Often, materials that exhibit those properties require large spin orbit coupling. We hypothesize that the emergent behavior can also occur due to spin, electron and phonon interactions in widely studied simple materials such as Si. That is, large intrinsic spin-orbit coupling is not an essential requirement for emergent behavior. The central hypothesis is that when one of the specimen dimensions is of the same order (or smaller) as the spin diffusion length, then non-equilibrium spin accumulation due to spin injection or spin-Hall effect (SHE) will lead to emergent phase transformations in the non-ferromagnetic semiconductors. In this experimental work, we report spin mediated emergent antiferromagnetism and metal insulator transition in a Pd (1 nm)/Ni81Fe19 (25 nm)/MgO (1 nm)/p-Si (~400 nm) thin film specimen. The spin-Hall effect in p-Si, observed through Rashba spin-orbit coupling mediated spin-Hall magnetoresistance behavior, is proposed to cause the spin accumulation and resulting emergent behavior. The phase transition is discovered from the diverging behavior in longitudinal third harmonic voltage, which is related to the thermal conductivity and heat capacity.

Control of entanglement transitions in quantum spin clusters

Science.gov (United States)

Irons, Hannah R.; Quintanilla, Jorge; Perring, Toby G.; Amico, Luigi; Aeppli, Gabriel

2017-12-01

Quantum spin clusters provide a platform for the experimental study of many-body entanglement. Here we address a simple model of a single-molecule nanomagnet featuring N interacting spins in a transverse field. The field can control an entanglement transition (ET). We calculate the magnetization, low-energy gap, and neutron-scattering cross section and find that the ET has distinct signatures, detectable at temperatures as high as 5% of the interaction strength. The signatures are stronger for smaller clusters.

Photo-modulation of the spin Hall conductivity of mono-layer transition metal dichalcogenides

Energy Technology Data Exchange (ETDEWEB)

Sengupta, Parijat; Bellotti, Enrico [Department of Electrical and Computer Engineering, Boston University, Boston, MA 02215 (United States)

2016-05-23

We report on a possible optical tuning of the spin Hall conductivity in mono-layer transition metal dichalcogenides. Light beams of frequencies much higher than the energy scale of the system (the off-resonant condition) do not excite electrons but rearrange the band structure. The rearrangement is quantitatively established using the Floquet formalism. For such a system of mono-layer transition metal dichalcogenides, the spin Hall conductivity (calculated with the Kubo expression in presence of disorder) exhibits a drop at higher frequencies and lower intensities. Finally, we compare the spin Hall conductivity of the higher spin-orbit coupled WSe{sub 2} to MoS{sub 2}; the spin Hall conductivity of WSe{sub 2} was found to be larger.

Large magnetoresistance dips and perfect spin-valley filter induced by topological phase transitions in silicene

Science.gov (United States)

Prarokijjak, Worasak; Soodchomshom, Bumned

2018-04-01

Spin-valley transport and magnetoresistance are investigated in silicene-based N/TB/N/TB/N junction where N and TB are normal silicene and topological barriers. The topological phase transitions in TB's are controlled by electric, exchange fields and circularly polarized light. As a result, we find that by applying electric and exchange fields, four groups of spin-valley currents are perfectly filtered, directly induced by topological phase transitions. Control of currents, carried by single, double and triple channels of spin-valley electrons in silicene junction, may be achievable by adjusting magnitudes of electric, exchange fields and circularly polarized light. We may identify that the key factor behind the spin-valley current filtered at the transition points may be due to zero and non-zero Chern numbers. Electrons that are allowed to transport at the transition points must obey zero-Chern number which is equivalent to zero mass and zero-Berry's curvature, while electrons with non-zero Chern number are perfectly suppressed. Very large magnetoresistance dips are found directly induced by topological phase transition points. Our study also discusses the effect of spin-valley dependent Hall conductivity at the transition points on ballistic transport and reveals the potential of silicene as a topological material for spin-valleytronics.

Effective coupling constants for spin-flip and non spin-flip E1 transitions in A--90 nuclei

International Nuclear Information System (INIS)

Nakayama, Shintaro; Shibata, Tokushi; Kishimoto, Tadafumi; Sasao, Mamiko; Ejiri, Hiroyasu

1983-01-01

Radiative proton capture reactions through two isobaric analogue resonances (IAR) in 89 Y were studied, one was the 12.07 MeV 2dsub(5/2) state lying just above the neutron threshold energy Bsub(n) and another was the 14.48 MeV 2dsub(3/2) state lying well above Bsub(n). E1 transitions from these IAR's were studied for favoured cases with no spin-flip and no change of radial nodes, and for unfavoured cases spin-flip and/or change of radial nodes. At the 2dsub(3/2) IAR lying well above Bsub(n), the favoured transitions show the resonance feature, but the unfavoured ones not. At the 2dsub(5/2) IAR near Bsub(n), however, both the favoured and unfavoured transitions show the resonance feature. Anormalous resonant feature of the unfavoured transitions is interpreted mainly due to the compound process. Favoured transitions are all found to be reduced by factors -- 0.3 over the shell model values. (author)

Control of the Speed of a Light-Induced Spin Transition through Mesoscale Core-Shell Architecture.

Science.gov (United States)

Felts, Ashley C; Slimani, Ahmed; Cain, John M; Andrus, Matthew J; Ahir, Akhil R; Abboud, Khalil A; Meisel, Mark W; Boukheddaden, Kamel; Talham, Daniel R

2018-05-02

The rate of the light-induced spin transition in a coordination polymer network solid dramatically increases when included as the core in mesoscale core-shell particles. A series of photomagnetic coordination polymer core-shell heterostructures, based on the light-switchable Rb a Co b [Fe(CN) 6 ] c · mH 2 O (RbCoFe-PBA) as core with the isostructural K j Ni k [Cr(CN) 6 ] l · nH 2 O (KNiCr-PBA) as shell, are studied using temperature-dependent powder X-ray diffraction and SQUID magnetometry. The core RbCoFe-PBA exhibits a charge transfer-induced spin transition (CTIST), which can be thermally and optically induced. When coupled to the shell, the rate of the optically induced transition from low spin to high spin increases. Isothermal relaxation from the optically induced high spin state of the core back to the low spin state and activation energies associated with the transition between these states were measured. The presence of a shell decreases the activation energy, which is associated with the elastic properties of the core. Numerical simulations using an electro-elastic model for the spin transition in core-shell particles supports the findings, demonstrating how coupling of the core to the shell changes the elastic properties of the system. The ability to tune the rate of optically induced magnetic and structural phase transitions through control of mesoscale architecture presents a new approach to the development of photoswitchable materials with tailored properties.

Quantum spin/valley Hall effect and topological insulator phase transitions in silicene

KAUST Repository

Tahir, M.

2013-04-26

We present a theoretical realization of quantum spin and quantum valley Hall effects in silicene. We show that combination of an electric field and intrinsic spin-orbit interaction leads to quantum phase transitions at the charge neutrality point. This phase transition from a two dimensional topological insulator to a trivial insulating state is accompanied by a quenching of the quantum spin Hall effect and the onset of a quantum valley Hall effect, providing a tool to experimentally tune the topological state of silicene. In contrast to graphene and other conventional topological insulators, the proposed effects in silicene are accessible to experiments.

Quantum spin/valley Hall effect and topological insulator phase transitions in silicene

KAUST Repository

Tahir, M.; Manchon, Aurelien; Sabeeh, K.; Schwingenschlö gl, Udo

2013-01-01

We present a theoretical realization of quantum spin and quantum valley Hall effects in silicene. We show that combination of an electric field and intrinsic spin-orbit interaction leads to quantum phase transitions at the charge neutrality point. This phase transition from a two dimensional topological insulator to a trivial insulating state is accompanied by a quenching of the quantum spin Hall effect and the onset of a quantum valley Hall effect, providing a tool to experimentally tune the topological state of silicene. In contrast to graphene and other conventional topological insulators, the proposed effects in silicene are accessible to experiments.

Unconventional transformation of spin Dirac phase across a topological quantum phase transition

Science.gov (United States)

Xu, Su-Yang; Neupane, Madhab; Belopolski, Ilya; Liu, Chang; Alidoust, Nasser; Bian, Guang; Jia, Shuang; Landolt, Gabriel; Slomski, Batosz; Dil, J. Hugo; Shibayev, Pavel P.; Basak, Susmita; Chang, Tay-Rong; Jeng, Horng-Tay; Cava, Robert J.; Lin, Hsin; Bansil, Arun; Hasan, M. Zahid

2015-01-01

The topology of a topological material can be encoded in its surface states. These surface states can only be removed by a bulk topological quantum phase transition into a trivial phase. Here we use photoemission spectroscopy to image the formation of protected surface states in a topological insulator as we chemically tune the system through a topological transition. Surprisingly, we discover an exotic spin-momentum locked, gapped surface state in the trivial phase that shares many important properties with the actual topological surface state in anticipation of the change of topology. Using a spin-resolved measurement, we show that apart from a surface bandgap these states develop spin textures similar to the topological surface states well before the transition. Our results offer a general paradigm for understanding how surface states in topological phases arise from a quantum phase transition and are suggestive for the future realization of Weyl arcs, condensed matter supersymmetry and other fascinating phenomena in the vicinity of a quantum criticality. PMID:25882717

Magnetization relaxation in spin glasses above transition point

International Nuclear Information System (INIS)

Zajtsev, I.A.; Minakov, A.A.; Galonzka, R.R.

1988-01-01

Magnetization relaxation of Cd 0.6 Zn 0.4 Cr 2 Se 4 and Cd 0.6 Mn 0.4 Te monocrystalline samples with T g =21 K and T g =12 K respectively and magnetic colloid is investigated. It is shown that magnetization inexponential relaxation detected experimentally in spin and dipole glasses is essentially higher than T g temperature transition. It is found that at temperatures higher than T g the essential difference is observed in behaviour of spin glasses with different Z and disorder types

Spin glass transition in canonical AuFe alloys: A numerical study

International Nuclear Information System (INIS)

Zhang, Kai-Cheng; Li, Yong-Feng; Liu, Gui-Bin; Zhu, Yan

2012-01-01

Although spin glass transitions have long been observed in diluted magnetic alloys, e.g. AuFe and CuMn alloys, previous numerical studies are not completely consistent with the experiment results. The abnormal critical exponents of the alloys remain still puzzling. By employing parallel tempering algorithm with finite-size scaling analysis, we investigated the phase transitions in canonical AuFe alloys. Our results strongly support that spin glass transitions occur at finite temperatures in the alloys. The calculated critical exponents agree well with those obtained from experiments. -- Highlights: ► By simulation we investigated the abnormal critical exponents observed in canonical SG alloys. ► The critical exponents obtained from our simulations agree well with those measured from experiments. ► Our results strongly support that RKKY interactions lead to SG transitions at finite temperatures.

Electronic structure and quantum spin fluctuations at the magnetic phase transition in MnSi

Science.gov (United States)

Povzner, A. A.; Volkov, A. G.; Nogovitsyna, T. A.

2018-05-01

The effect of spin fluctuations on the heat capacity and homogeneous magnetic susceptibility of the chiral magnetic MnSi in the vicinity of magnetic transition has been investigated by using the free energy functional of the coupled electron and spin subsystems and taking into account the Dzyaloshinsky-Moriya interaction. For helical ferromagnetic ordering, we found that zero-point fluctuations of the spin density are large and comparable with fluctuations of the non-uniform magnetization. The amplitude of zero-point spin fluctuations shows a sharp decrease in the region of the magnetic phase transition. It is shown that sharp decrease of the amplitude of the quantum spin fluctuations results in the lambda-like maxima of the heat capacity and the homogeneous magnetic susceptibility. Above the temperature of the lambda anomaly, the spin correlation radius becomes less than the period of the helical structure and chiral fluctuations of the local magnetization appear. It is shown that formation of a "shoulder" on the temperature dependence of the heat capacity is due to disappearance of the local magnetization. Our finding allows to explain the experimentally observed features of the magnetic phase transition of MnSi as a result of the crossover of quantum and thermodynamic phase transitions.

Abnormal Elasticity of Single-Crystal Magnesiosiderite across the Spin Transition in Earth's Lower Mantle

Science.gov (United States)

Fu, Suyu; Yang, Jing; Lin, Jung-Fu

2017-01-01

Brillouin light scattering and impulsive stimulated light scattering have been used to determine the full elastic constants of magnesiosiderite [(Mg0.35Fe0.65)CO3 ] up to 70 GPa at room temperature in a diamond-anvil cell. Drastic softening in C11 , C33 , C12 , and C13 elastic moduli associated with the compressive stress component and stiffening in C44 and C14 moduli associated with the shear stress component are observed to occur within the spin transition between ˜42.4 and ˜46.5 GPa . Negative values of C12 and C13 are also observed within the spin transition region. The Born criteria constants for the crystal remain positive within the spin transition, indicating that the mixed-spin state remains mechanically stable. Significant auxeticity can be related to the electronic spin transition-induced elastic anomalies based on the analysis of Poisson's ratio. These elastic anomalies are explained using a thermoelastic model for the rhombohedral system. Finally, we conclude that mixed-spin state ferromagnesite, which is potentially a major deep-carbon carrier, is expected to exhibit abnormal elasticity, including a negative Poisson's ratio of -0.6 and drastically reduced VP by 10%, in Earth's midlower mantle.

Evidence for a pressure-induced spin transition in olivine-type LiFePO4 triphylite

Science.gov (United States)

Núñez Valdez, Maribel; Efthimiopoulos, Ilias; Taran, Michail; Müller, Jan; Bykova, Elena; McCammon, Catherine; Koch-Müller, Monika; Wilke, Max

2018-05-01

We present a combination of first-principles and experimental results regarding the structural and magnetic properties of olivine-type LiFePO4 under pressure. Our investigations indicate that the starting P b n m phase of LiFePO4 persists up to 70 GPa. Further compression leads to an isostructural transition in the pressure range of 70-75 GPa, inconsistent with a former theoretical study. Considering our first-principles prediction for a high-spin to low-spin transition of Fe2 + close to 72 GPa, we attribute the experimentally observed isostructural transition to a change in the spin state of Fe2 + in LiFePO4. Compared to relevant Fe-bearing minerals, LiFePO4 exhibits the largest onset pressure for a pressure-induced spin state transition.

Quantum phase transitions in matrix product states of one-dimensional spin-1 chains

International Nuclear Information System (INIS)

Zhu Jingmin

2014-01-01

We present a new model of quantum phase transitions in matrix product systems of one-dimensional spin-1 chains and study the phases coexistence phenomenon. We find that in the thermodynamic limit the proposed system has three different quantum phases and by adjusting the control parameters we are able to realize any phase, any two phases equal coexistence and the three phases equal coexistence. At every critical point the physical quantities including the entanglement are not discontinuous and the matrix product system has long-range correlation and N-spin maximal entanglement. We believe that our work is helpful for having a comprehensive understanding of quantum phase transitions in matrix product states of one-dimensional spin chains and of certain directive significance to the preparation and control of one-dimensional spin lattice models with stable coherence and N-spin maximal entanglement. (author)

Reorientation effects for 52 MeV vector polarized deuterons

International Nuclear Information System (INIS)

Nurzynski, J.; Kihm, T.; Knopfle, K.T.; Mairle, G.; Clement, H.

1987-01-01

The differential cross sections and the vector analysing powers were measured for the elastic and inelastic scattering of 52 MeV vector polarized deuterons from 20 Ne, 22 Ne, 26 Mg, 28 Si, 32 S, 34 S, 36 Ar and 40 Ar nuclei. Coupled channels analysis was carried out using an axially symmetric rotational model with either prolate or oblate quadrupole deformations for each isotope. Calculations assuming harmonic vibrator model were also carried out. In general, reorientation effects were found to be weak. A global optical model potential containing an imaginary spin-orbit component was found to be the most suitable in describing the experimental data at this energy

Optimal Charge-to-Spin Conversion in Graphene on Transition-Metal Dichalcogenides

Science.gov (United States)

Offidani, Manuel; Milletarı, Mirco; Raimondi, Roberto; Ferreira, Aires

2017-11-01

When graphene is placed on a monolayer of semiconducting transition metal dichalcogenide (TMD) its band structure develops rich spin textures due to proximity spin-orbital effects with interfacial breaking of inversion symmetry. In this work, we show that the characteristic spin winding of low-energy states in graphene on a TMD monolayer enables current-driven spin polarization, a phenomenon known as the inverse spin galvanic effect (ISGE). By introducing a proper figure of merit, we quantify the efficiency of charge-to-spin conversion and show it is close to unity when the Fermi level approaches the spin minority band. Remarkably, at high electronic density, even though subbands with opposite spin helicities are occupied, the efficiency decays only algebraically. The giant ISGE predicted for graphene on TMD monolayers is robust against disorder and remains large at room temperature.

Enhanced spin accumulation in Fe3O4 based spin injection devices below the Verwey transition

Science.gov (United States)

Bhat, Shwetha G.; Kumar, P. S. Anil

2016-12-01

Spin injection into GaAs and Si (both n and p-type) semiconductors using Fe3O4 is achieved with and without a tunnel barrier (MgO) via three-terminal electrical Hanle measurement. Interestingly, the magnitude of spin accumulation voltage (ΔV) in semiconductor is found to be associated with a drastic increment in ΔV in Fe3O4 based devices for temperature metal-to-insulator transition of Fe3O4 at T V. Observations from our elaborate investigations show that spin polarization of Fe3O4 has an explicit influence on the enhanced spin injection. It is argued that the theoretical prediction of half-metallicity of Fe3O4 above and below T V has to be reinvestigated.

Phase transitions and thermal entanglement of the distorted Ising-Heisenberg spin chain: topology of multiple-spin exchange interactions in spin ladders

Science.gov (United States)

Arian Zad, Hamid; Ananikian, Nerses

2017-11-01

We consider a symmetric spin-1/2 Ising-XXZ double sawtooth spin ladder obtained from distorting a spin chain, with the XXZ interaction between the interstitial Heisenberg dimers (which are connected to the spins based on the legs via an Ising-type interaction), the Ising coupling between nearest-neighbor spins of the legs and rungs spins, respectively, and additional cyclic four-spin exchange (ring exchange) in the square plaquette of each block. The presented analysis supplemented by results of the exact solution of the model with infinite periodic boundary implies a rich ground state phase diagram. As well as the quantum phase transitions, the characteristics of some of the thermodynamic parameters such as heat capacity, magnetization and magnetic susceptibility are investigated. We prove here that among the considered thermodynamic and thermal parameters, solely heat capacity is sensitive versus the changes of the cyclic four-spin exchange interaction. By using the heat capacity function, we obtain a singularity relation between the cyclic four-spin exchange interaction and the exchange coupling between pair spins on each rung of the spin ladder. All thermal and thermodynamic quantities under consideration should be investigated by regarding those points which satisfy the singularity relation. The thermal entanglement within the Heisenberg spin dimers is investigated by using the concurrence, which is calculated from a relevant reduced density operator in the thermodynamic limit.

Tuning magnetoresistance in molybdenum disulphide and graphene using a molecular spin transition.

Science.gov (United States)

Datta, Subhadeep; Cai, Yongqing; Yudhistira, Indra; Zeng, Zebing; Zhang, Yong-Wei; Zhang, Han; Adam, Shaffique; Wu, Jishan; Loh, Kian Ping

2017-09-22

Coupling spins of molecular magnets to two-dimensional (2D) materials provides a framework to manipulate the magneto-conductance of 2D materials. However, with most molecules, the spin coupling is usually weak and devices fabricated from these require operation at low temperatures, which prevents practical applications. Here, we demonstrate field-effect transistors based on the coupling of a magnetic molecule quinoidal dithienyl perylenequinodimethane (QDTP) to 2D materials. Uniquely, QDTP switches from a spin-singlet state at low temperature to a spin-triplet state above 370 K, and the spin transition can be electrically transduced by both graphene and molybdenum disulphide. Graphene-QDTP shows hole-doping and a large positive magnetoresistance ( ~ 50%), while molybdenum disulphide-QDTP demonstrates electron-doping and a switch to large negative magnetoresistance ( ~ 100%) above the magnetic transition. Our work shows the promise of spin detection at high temperature by coupling 2D materials and molecular magnets.Engineering a coupling between magnetic molecules and conducting materials at room temperature could help the development of spintronic devices. Loh et al. show that the spin state of QDTP molecules deposited on graphene and MoS 2 couples to their electronic structure, affecting magnetotransport.

Change of cobalt magnetic anisotropy and spin polarization with alkanethiolates self-assembled monolayers

International Nuclear Information System (INIS)

Campiglio, Paolo; Breitwieser, Romain; Repain, Vincent; Guitteny, Solène; Chacon, Cyril; Bellec, Amandine; Lagoute, Jérôme; Girard, Yann; Rousset, Sylvie; Sassella, Adele; Imam, Mighfar; Narasimhan, Shobhana

2015-01-01

We demonstrate that the deposition of a self-assembled monolayer of alkanethiolates on a 1 nm thick cobalt ultrathin film grown on Au(111) induces a spin reorientation transition from in-plane to out-of-plane magnetization. Using ab initio calculations, we show that a methanethiolate layer changes slightly both the magnetocrystalline and shape anisotropy, both effects almost cancelling each other out for a 1 nm Co film. Finally, the change in hysteresis cycles upon alkanethiolate adsorption could be assigned to a molecular-induced roughening of the Co layer, as shown by STM. In addition, we calculate how a methanethiolate layer modifies the spin density of states of the Co layer and we show that the spin polarization at the Fermi level through the organic layer is reversed as compared to the uncovered Co. These results give new theoretical and experimental insights for the use of thiol-based self-assembled monolayers in spintronic devices. (paper)

Unambiguously identifying spin states of transition-metal ions in the Earth (Invited)

Science.gov (United States)

Hsu, H.

2010-12-01

The spin state of a transition-metal ion in crystalline solids, defined by the number of unpaired electrons in the ion’s incomplete 3d shell, may vary with many factors, such as temperature, pressure, strain, and the local atomic configuration, to name a few. Such a phenomenon, known as spin-state crossover, plays a crucial role in spintronic materials. Recently, the pressure-induced spin-state crossover in iron-bearing minerals has been recognized to affect the minerals’ structural and elastic properties. However, the detailed mechanism of such crossover in iron-bearing magnesium silicate perovskite, the most abundant mineral in the Earth, remains unclear. A significant part of this confusion arises from the difficulty in reliably extracting the spin state from experiments. For the same reason, the thermally-induced spin-state crossover in lanthanum cobaltite (LaCoO3) has been controversial for more than four decades. In this talk, I will discuss how first-principle calculations can help clarifying these long-standing controversies. In addition to the total energy, equation of state, and elastic properties of each spin state, first-principle calculations also predict the electric field gradient (EFG) at the nucleus of each transition-metal ion. Our calculations showed that the nuclear EFG, a quantity that can be measured via Mössbauer or nuclear magnetic resonance (NMR) spectroscopy, depends primarily on the spin state, irrespective of the concentration or configuration of transition-metal ions. Such robustness makes EFG a unique fingerprint to identify the spin state. The combination of first-principle calculations and Mössbauer/NMR spectroscopy can therefore be a reliable and efficient approach in tackling spin-state crossover problems in the Earth. This work was primarily supported by the MRSEC Program of NSF under Awards Number DMR-0212302 and DMR-0819885, and partially supported by NSF under ATM-0428774 (V-Lab), EAR-1019853, and EAR-0810272. The

Phase transitions and multicritical points in the mixed spin-32 and spin-2 Ising system with a single-ion anisotropy

International Nuclear Information System (INIS)

Bobak, A.; Dely, J.

2007-01-01

The effect of a single-ion anisotropy on the phase diagram of the mixed spin-32 and spin-2 Ising system is investigated by the use of a mean-field theory based on the Bogoliubov inequality for the free energy. Topologically different kinds of phase diagrams are achieved by changing values of the parameter in the model Hamiltonian. Besides second-order transitions, lines of first-order transitions terminating either at a tricritical point or an isolated critical point, are found

Spin delocalization phase transition in a correlated electrons model

International Nuclear Information System (INIS)

Huerta, L.

1990-11-01

In a simplified one-site model for correlated electrons systems we show the existence of a phase transition corresponding to spin delocalization. The system becomes a solvable model and zero-dimensional functional techniques are used. (author). 7 refs, 3 figs

Spin Chern number and topological phase transition on the Lieb lattice with spin–orbit coupling

International Nuclear Information System (INIS)

Chen, Rui; Zhou, Bin

2017-01-01

We propose that quantum anomalous Hall effect may occur in the Lieb lattice, when Rashba spin–orbit coupling, spin-independent and spin-dependent staggered potentials are introduced into the lattice. It is found that spin Chern numbers of two degenerate flat bands change from 0 to ±2 due to Rashba spin–orbit coupling effect. The inclusion of Rashba spin–orbit coupling and two kinds of staggered potentials opens a gap between the two flat bands. The topological property of the gap is determined by the amplitudes of Rashba spin–orbit coupling and staggered potentials, and thus the topological phase transition from quantum anomalous Hall effect to normal insulator can occur. Finally, the topological phase transition from quantum spin Hall state to normal insulator is discussed when Rashba spin–orbit coupling and intrinsic spin–orbit coupling coexist in the Lieb lattice. - Highlights: • Spin Chern numbers of the bulk states on the Lieb lattice are calculated. • RSOC plays an important role on the topological phase transition on the Lieb lattice. • Quantum anomalous Hall effect can occur due to RSOC and staggered potentials. • Topological phase transition can occur when ISOC and RSOC coexist.

Spin relaxation and the Kondo effect in transition metal dichalcogenide monolayers

International Nuclear Information System (INIS)

Rostami, Habib; Moghaddam, Ali G; Asgari, Reza

2016-01-01

We investigate the spin relaxation and Kondo resistivity caused by magnetic impurities in doped transition metal dichalcogenide monolayers. We show that momentum and spin relaxation times, due to the exchange interaction by magnetic impurities, are much longer when the Fermi level is inside the spin-split region of the valence band. In contrast to the spin relaxation, we find that the dependence of Kondo temperature T K on the doping is not strongly affected by the spin–orbit induced splitting, although only one of the spin species are present at each valley. This result, which is obtained using both perturbation theory and the poor man’s scaling methods, originates from the intervalley spin-flip scattering in the spin-split region. We further demonstrate the decline in the conductivity with temperatures close to T K , which can vary with the doping. Our findings reveal the qualitative difference with the Kondo physics in conventional metallic systems and other Dirac materials. (paper)

Topological quantum phase transitions and edge states in spin-orbital coupled Fermi gases.

Science.gov (United States)

Zhou, Tao; Gao, Yi; Wang, Z D

2014-06-11

We study superconducting states in the presence of spin-orbital coupling and Zeeman field. It is found that a phase transition from a Fulde-Ferrell-Larkin-Ovchinnikov state to the topological superconducting state occurs upon increasing the spin-orbital coupling. The nature of this topological phase transition and its critical property are investigated numerically. Physical properties of the topological superconducting phase are also explored. Moreover, the local density of states is calculated, through which the topological feature may be tested experimentally.

Successes of trade reorientation and expansion in post-communist transition: an enterprise-level approach

Directory of Open Access Journals (Sweden)

Jan Winiecki

2000-06-01

Full Text Available The article offers an approach to the westward reorientation of foreign trade by the post-communist economies of East-Central Europe at the micro--i.e. enterprise--level. Having presented the dynamics of reorientation and its theoretical/historical underpinnings, the writer then goes on to underline the surprisingly large number of microeconomic determinants behind the strong westbound export surge. The article starts with the most often cited factor, namely the distressed sale argument, and then shifts the focus to determinants that have received far less attention: an unusual extension of the "distressed sale" argument and another, more important one, namely the legacy of the oversized industrial sector and resultant availability of firms ready (or forced to test their mettle on the world markets. The following section extends the list of determinants to foreign direct investment and the growing export activity of domestic de novo firms. The linkages between the determinants are also pointed out. The final section sums up the observations.

Long Spin-Relaxation Times in a Transition-Metal Atom in Direct Contact to a Metal Substrate.

Science.gov (United States)

Hermenau, Jan; Ternes, Markus; Steinbrecher, Manuel; Wiesendanger, Roland; Wiebe, Jens

2018-03-14

Long spin-relaxation times are a prerequisite for the use of spins in data storage or nanospintronics technologies. An atomic-scale solid-state realization of such a system is the spin of a transition-metal atom adsorbed on a suitable substrate. For the case of a metallic substrate, which enables the direct addressing of the spin by conduction electrons, the experimentally measured lifetimes reported to date are on the order of only hundreds of femtoseconds. Here, we show that the spin states of iron atoms adsorbed directly on a conductive platinum substrate have a surprisingly long spin-relaxation time in the nanosecond regime, which is comparable to that of a transition metal atom decoupled from the substrate electrons by a thin decoupling layer. The combination of long spin-relaxation times and strong coupling to conduction electrons implies the possibility to use flexible coupling schemes to process the spin information.

Nuclear shape transitions and some properties of aligned-particle configurations at high spin

International Nuclear Information System (INIS)

Koo, T.L.; Chowdhury, P.; Emling, H.

1982-01-01

Two topics are addressed in this paper. First, we discuss the variation of shapes with spin and neutron number for nuclei in the N approx. = 88 transitional region. Second, we present comments on the feeding times of very high spin single-particle yrast states

Reorienting with terrain slope and landmarks.

Science.gov (United States)

Nardi, Daniele; Newcombe, Nora S; Shipley, Thomas F

2013-02-01

Orientation (or reorientation) is the first step in navigation, because establishing a spatial frame of reference is essential for a sense of location and heading direction. Recent research on nonhuman animals has revealed that the vertical component of an environment provides an important source of spatial information, in both terrestrial and aquatic settings. Nonetheless, humans show large individual and sex differences in the ability to use terrain slope for reorientation. To understand why some participants--mainly women--exhibit a difficulty with slope, we tested reorientation in a richer environment than had been used previously, including both a tilted floor and a set of distinct objects that could be used as landmarks. This environment allowed for the use of two different strategies for solving the task, one based on directional cues (slope gradient) and one based on positional cues (landmarks). Overall, rather than using both cues, participants tended to focus on just one. Although men and women did not differ significantly in their encoding of or reliance on the two strategies, men showed greater confidence in solving the reorientation task. These facts suggest that one possible cause of the female difficulty with slope might be a generally lower spatial confidence during reorientation.

Large isosymmetric reorientation of oxygen octahedra rotation axes in epitaxially strained perovskites.

Science.gov (United States)

Rondinelli, James M; Coh, Sinisa

2011-06-10

Using first-principles density functional theory calculations, we discover an anomalously large biaxial strain-induced octahedral rotation axis reorientation in orthorhombic perovskites with tendency towards rhombohedral symmetry. The transition between crystallographically equivalent (isosymmetric) structures with different octahedral rotation magnitudes originates from strong strain-octahedral rotation coupling available to perovskites and the energetic hierarchy among competing octahedral tilt patterns. By elucidating these criteria, we suggest many functional perovskites would exhibit the transition in thin film form, thus offering a new landscape in which to tailor highly anisotropic electronic responses.

Magnetic phase transitions and magnetization reversal in MnRuP

Science.gov (United States)

Lampen-Kelley, P.; Mandrus, D.

The ternary phosphide MnRuP is an incommensurate antiferromagnetic metal crystallizing in the non-centrosymmetric Fe2P-type crystal structure. Below the Neel transition at 250 K, MnRuP exhibits hysteretic anomalies in resistivity and magnetic susceptibility curves as the propagation vectors of the spiral spin structure change discontinuously across T1 = 180 K and T2 = 100 K. Temperature-dependent X-ray diffraction data indicate that the first-order spin reorientation occurs in the absence of a structural transition. A strong magnetization reversal (MR) effect is observed upon cooling the system through TN in moderate dc magnetic fields. Positive magnetization is recovered on further cooling through T1 and maintained in subsequent warming curves. The field dependence and training of the MR effect in MnRuP will be discussed in terms of the underlying magnetic structures and compared to anomalous MR observed in vanadate systems. This work is supported by the Gordon and Betty Moore Foundation GBMF4416 and U.S. DOE, Office of Science, BES, Materials Science and Engineering Division.

Glass transition in the spin-density wave phase of (TMTSF)2PF6

DEFF Research Database (Denmark)

Lasjaunias, J.C.; Biljakovic, K.; Nad, F.

1994-01-01

We present the results of low frequency dielectric measurements and a detailed kinetic investigation of the specific heat anomaly in the spin-density wave phase of (TMTSF)(2)PF6 in the temperature range between 2 and 4 K. The dielectric relaxation shows a critical slowing down towards a ''static'......'' glass transition around 2 K. The jump in the specific heat in different controlled kinetic conditions shows all the characteristics of freezing in supercooled liquids. Both effects give direct evidence of a glass transition in the spin-density wave ground state....

Magnetic phase transitions in low dimension quantum spin systems

International Nuclear Information System (INIS)

Canevet, Emmanuel

2010-01-01

In this PhD thesis, three low dimensional spin systems are studied by means of elastic and inelastic neutron scattering. Macroscopic measurements in the DMACuCl 3 compound indicate the coexistence of two kinds of dimers: antiferromagnetic and ferromagnetic. The magnetic structure determined by our neutron diffraction survey at H = 0 shows irrevocably the existence of these two kinds of dimers. It has been shown that the Ising-like compound BaCo 2 V 2 O 8 should be the first realization of a system in which a longitudinal spin density wave (LSDW) magnetic order occurs when a magnetic field is applied. In a first time, we have determined the magnetic structure in zero magnetic field. Then, we focused on the effect of a magnetic field on the propagation vector, showing an entrance in the LSDW phase at H c = 3.9 T. The magnetic structure refined above this critical field confirms that BaCo 2 V 2 O 8 is the first compound in which occurs a LSDW phase. In the organic compound DF 5 PNN, it has been shown that this compound is well described at low temperature by spin chains with alternating couplings. However, the crystallographic structure determined at room temperature implies that the interactions are uniform. By means of neutron diffraction, we characterized a structural transition at low temperature (T c = 450 mK) making the system evolve from C2/c space group to Pc. This transition explains the alternating behavior of the interactions. We have also evidenced a field-induced structural transition (H c = 1.1 T). Above this field, the system is back to the C2/c space group, implying that the interactions are back to uniform. We have confirmed this by studying the magnetic excitations. (author) [fr

Calculation of the magnetic anisotropy energy and finite-temperature magnetic properties of transition-metal films

International Nuclear Information System (INIS)

Garibay-Alonso, R; Villasenor-Gonzalez, P; Dorantes-Davila, J; Pastor, G M

2004-01-01

The magnetic anisotropy energy at the interface (IMAE) of Co films deposited on the Pd(111) surface are determined in the framework of a self-consistent, real-space tight-binding method at zero temperature. Significant spin moments are induced at the Pd atoms at the interface which have an important influence on the observed reorientation transitions as a function of Co film thickness. Film-substrate hybridizations are therefore crucial for the magneto-anisotropic behaviour of thin transition-metal films deposited on metallic non-magnetic substrates. Furthermore, using a real-space recursive expansion of the local Green function and within the virtual-crystal approximation we calculate the magnetization curves and the Curie temperature T C for free-standing Fe films

Noise as a Probe of Ising Spin Glass Transitions

Science.gov (United States)

Chen, Zhi; Yu, Clare

2009-03-01

Noise is ubiquitous and and is often viewed as a nuisance. However, we propose that noise can be used as a probe of the fluctuations of microscopic entities, especially in the vicinity of a phase transition. In recent work we have used simulations to show that the noise increases in the vicinity of phase transitions of ordered systems. We have recently turned our attention to noise near the phase transitions of disordered systems. In particular, we are studying the noise near Ising spin glass transitions using Monte Carlo simulations. We monitor the system as a function of temperature. At each temperature, we obtain the time series of quantities characterizing the properties of the system, i.e., the energy and magnetization. We look at different quantities, such as the noise power spectrum and the second spectrum of the noise, to analyze the fluctuations.

A study of stress reorientation of hydrides in zircaloy

Energy Technology Data Exchange (ETDEWEB)

Yourong, Jiang; Bangxin, Zhou [Nuclear Power Inst. of China, Chengdu, SC (China)

1994-10-01

Under the conditions of circumferential tensile stress from 70 to 180 MPa for Zircaloy tubes or the tensile stress from 55 to 180 MPa for Zircaloy-4 plates and temperature cycling between 150 and 400 degree C, the effects of stress and the number of temperature cycling on hydride reorientation in Zircaloy-4 tubes and plates and Zircaloy-2 tubes containing about 220 {mu}g/g hydrogen have been investigated. With the increase of stress and/or the number of temperature cycling, the level of hydride reorientation increases. When hydride reorientation takes place, there is a threshold stress concerned with the number of temperature cycling. Below the threshold stress, hydride reorientation is not obvious. When applied stress is higher than the threshold stress, the level of hydride reorientation increases with the increase of stress and the number of temperature cycling. Hydride reorientation in Zircaloy-4 tubes develops gradually from the outer surface to inner surface. It might be related to the difference of texture between outer surface and inner surface. The threshold stress is affected by both the texture and the value of B. So controlling texture could still restrict hydride reorientation under tensile stress.

Effect of Spin Transition onComposition and Seismic Structure of the Lower Mantle

Science.gov (United States)

Wu, Z.

2015-12-01

Spin transition of iron in ferropericlase (Fp) causes a significant softening in bulk modulus [e.g.,1,2], which leads to unusual dVP/dT>0. Because dVP/dT>0 in Fp cancels out with dVP/dTMao, Z., Marquardt, H., 2013. . Rev Geophys 51, 244-275 (2013). [3] Wu, Z.Q., Wentzcovitch, R.M., 2014. Spin crossover in ferropericlase and velocity heterogeneities in the lower mantle. Proc. Natl. Acad. Sci. U. S. A. 111, 10468-10472. [4] Zhao, D.P., 2007. Seismic images under 60 hotspots: Search for mantle plumes. Gondwana Res 12, 335-355. [5] van der Hilst, R.D., Karason, H., 1999. Science 283, 1885-1888. [6] Huang,C., Leng, W., Wu, Z. Q., 2015. Iron-spin transition controls structure and stability of LLSVPs in the lower mantle, Earth Planet. Sci. Lett. 423, 173-181.

Exact-exchange spin-density functional theory of Wigner localization and phase transitions in quantum rings.

Science.gov (United States)

Arnold, Thorsten; Siegmund, Marc; Pankratov, Oleg

2011-08-24

We apply exact-exchange spin-density functional theory in the Krieger-Li-Iafrate approximation to interacting electrons in quantum rings of different widths. The rings are threaded by a magnetic flux that induces a persistent current. A weak space and spin symmetry breaking potential is introduced to allow for localized solutions. As the electron-electron interaction strength described by the dimensionless parameter r(S) is increased, we observe-at a fixed spin magnetic moment-the subsequent transition of both spin sub-systems from the Fermi liquid to the Wigner crystal state. A dramatic signature of Wigner crystallization is that the persistent current drops sharply with increasing r(S). We observe simultaneously the emergence of pronounced oscillations in the spin-resolved densities and in the electron localization functions indicating a spatial electron localization showing ferrimagnetic order after both spin sub-systems have undergone the Wigner crystallization. The critical r(S)(c) at the transition point is substantially smaller than in a fully spin-polarized system and decreases further with decreasing ring width. Relaxing the constraint of a fixed spin magnetic moment, we find that on increasing r(S) the stable phase changes from an unpolarized Fermi liquid to an antiferromagnetic Wigner crystal and finally to a fully polarized Fermi liquid. © 2011 IOP Publishing Ltd

Spin transition diagram of (2Me-5Et-PyH)[Fe(Th-5Cl-Sa)2] studied by EPR

International Nuclear Information System (INIS)

Krupska, A.; Augustyniak-Jablokow, M.A.; Yablokov, V.Yu.; Zelentsov, V.V.

2005-01-01

The high-spin - low-spin transition in (2Me-5Et-PyH)[Fe(Th-5Cl-Sa) 2 ] was studied by EPR under hydrostatic pressure in the temperature range of 80-310 K. Two modifications of the low-spin complexes: low-pressure (LS-1) and high-pressure (S-2) ones were observed. The low-spin complexes are associated in domains. Under atmospheric pressure LS-1 appears or disappears at 220 K. The hydrostatic pressure shifts the transition to high temperatures. Above 410 MPa the abrupt changes of the g-factor and width ΔB of the EPR line is observed. The pressure-induced transition LS-1 - LS-2 is almost independent of T up to 275 K where under pressure 420 MPa a triple point is observed. When the pressure has been decreased the reverse transition from LS-2 to LS-1 or to high spin phase (at T > 260 K) occurs with a large hysteresis about 95 MPa. (author)

2-vertex Lorentzian spin foam amplitudes for dipole transitions

Science.gov (United States)

Sarno, Giorgio; Speziale, Simone; Stagno, Gabriele V.

2018-04-01

We compute transition amplitudes between two spin networks with dipole graphs, using the Lorentzian EPRL model with up to two (non-simplicial) vertices. We find power-law decreasing amplitudes in the large spin limit, decreasing faster as the complexity of the foam increases. There are no oscillations nor asymptotic Regge actions at the order considered, nonetheless the amplitudes still induce non-trivial correlations. Spin correlations between the two dipoles appear only when one internal face is present in the foam. We compute them within a mini-superspace description, finding positive correlations, decreasing in value with the Immirzi parameter. The paper also provides an explicit guide to computing Lorentzian amplitudes using the factorisation property of SL(2,C) Clebsch-Gordan coefficients in terms of SU(2) ones. We discuss some of the difficulties of non-simplicial foams, and provide a specific criterion to partially limit the proliferation of diagrams. We systematically compare the results with the simplified EPRLs model, much faster to evaluate, to learn evidence on when it provides reliable approximations of the full amplitudes. Finally, we comment on implications of our results for the physics of non-simplicial spin foams and their resummation.

Single crystal growth, magnetic and thermal properties of perovskite YFe{sub 0.6}Mn{sub 0.4}O{sub 3} single crystal

Energy Technology Data Exchange (ETDEWEB)

Xie, Tao [School of Materials Science and Engineering, Shanghai Institute of Technology, Shanghai 201418 (China); Synthetio Single Crystal Research Center, Shanghai Institute of Ceramic, Chinese Academy of Sciences, Shanghai 200050 (China); Key Laboratory of Transparent and Opto-functional Inorganic Materials, Shanghai Institute of Ceramics, Chinese Academy of Sciences, Shanghai 200050 (China); Shen, Hui, E-mail: hshen@sit.edu.cn [School of Materials Science and Engineering, Shanghai Institute of Technology, Shanghai 201418 (China); Zhao, Xiangyang; Man, Peiwen [Synthetio Single Crystal Research Center, Shanghai Institute of Ceramic, Chinese Academy of Sciences, Shanghai 200050 (China); Key Laboratory of Transparent and Opto-functional Inorganic Materials, Shanghai Institute of Ceramics, Chinese Academy of Sciences, Shanghai 200050 (China); Wu, Anhua, E-mail: wuanhua@mail.sic.ac.cn [Synthetio Single Crystal Research Center, Shanghai Institute of Ceramic, Chinese Academy of Sciences, Shanghai 200050 (China); Key Laboratory of Transparent and Opto-functional Inorganic Materials, Shanghai Institute of Ceramics, Chinese Academy of Sciences, Shanghai 200050 (China); Su, Liangbi [Synthetio Single Crystal Research Center, Shanghai Institute of Ceramic, Chinese Academy of Sciences, Shanghai 200050 (China); Key Laboratory of Transparent and Opto-functional Inorganic Materials, Shanghai Institute of Ceramics, Chinese Academy of Sciences, Shanghai 200050 (China); Xu, Jiayue, E-mail: xujiayue@sit.edu.cn [School of Materials Science and Engineering, Shanghai Institute of Technology, Shanghai 201418 (China)

2016-11-01

High quality YFe{sub 0.6}Mn{sub 0.4}O{sub 3} single crystal was grown by floating zone technique using a four-mirror-image-furnace under flowing air. Powder X-ray diffraction gives well evidence that the specimen has an orthorhombic structure, with space group Pbnm. Temperature dependence of the magnetizations of YFe{sub 0.6}Mn{sub 0.4}O{sub 3} single crystal were studied under ZFC and FC modes in the temperature range from 5 K to 400 K. A clear spin reorientation transition behavior (Γ{sub 4}→Γ{sub 1}) is observed in the temperature range of 322–316 K, due to the substitution of Mn at the Fe site of YFeO{sub 3}. Its Néel temperature is around 385 K. Moreover, the spin reorientation is verified by the change of magnetic hysteresis loops of the sample along [001] axis in the temperature range of 50–385 K. The thermal properties of the sample were measured by the differential scanning calorimeter (DSC) from 300 K to 500 K, which also clearly appear anomaly in the spin reorientation region. - Highlights: • High quality YFe{sub 0.6}Mn{sub 0.4}O{sub 3} single crystal was grown by floating zone technique. • The thermal properties appear anomaly in the spin reorientation region. • A clear spin reorientation transition behavior (Γ{sub 4}→Γ{sub 1}) is observed in the temperature range of 322–316 K, due to the substitution of Mn at the Fe site of YFeO{sub 3}.

Smoothed transitions in higher spin AdS gravity

International Nuclear Information System (INIS)

Banerjee, Shamik; Shenker, Stephen; Castro, Alejandra; Hellerman, Simeon; Hijano, Eliot; Lepage-Jutier, Arnaud; Maloney, Alexander

2013-01-01

We consider CFTs conjectured to be dual to higher spin theories of gravity in AdS 3 and AdS 4 . Two-dimensional CFTs with W N symmetry are considered in the λ = 0 (k → ∞) limit where they are conjectured to be described by continuous orbifolds. The torus partition function is computed, using reasonable assumptions, and equals that of a free-field theory. We find no phase transition at temperatures of order 1; the usual Hawking–Page phase transition is removed by the highly degenerate light states associated with conical defect states in the bulk. Three-dimensional Chern–Simons matter CFTs with vector-like matter are considered on T 3 , where the dynamics is described by an effective theory for the eigenvalues of the holonomies. Likewise, we find no evidence for a Hawking–Page phase transition at a large level k. (paper)

Dynamical phase transitions in spin models and automata

International Nuclear Information System (INIS)

Derrida, B.

1989-01-01

Some of the models and methods developed in the study of the dynamics of spin models and automata are described. Special attention is given to the distance method which consists of comparing the time evolution of two configurations. The method is used to obtain the phase boundary between a frozen and a chaotic phase in the case of deterministic models. For stochastic systems the method is used to obtain dynamical phase transitions

Analytical evidence for the absence of spin glass transition on self-dual lattices

International Nuclear Information System (INIS)

Ohzeki, Masayuki; Nishimori, Hidetoshi

2009-01-01

We show strong evidence for the absence of a finite-temperature spin glass transition for the random-bond Ising model on self-dual lattices. The analysis is performed by an application of duality relations, which enables us to derive a precise but approximate location of the multicritical point on the Nishimori line. This method can be systematically improved to presumably give the exact result asymptotically. The duality analysis, in conjunction with the relationship between the multicritical point and the spin glass transition point for the symmetric distribution function of randomness, leads to the conclusion of the absence of a finite-temperature spin glass transition for the case of symmetric distribution. The result is applicable to the random-bond Ising model with ±J or Gaussian distribution and the Potts gauge glass on the square, triangular and hexagonal lattices as well as the random three-body Ising model on the triangular and the Union-Jack lattices and the four-dimensional random plaquette gauge model. This conclusion is exact provided that the replica method is valid and the asymptotic limit of the duality analysis yields the exact location of the multicritical point. (fast track communication)

Phase Transitions in Definite Total Spin States of Two-Component Fermi Gases.

Science.gov (United States)

Yurovsky, Vladimir A

2017-05-19

Second-order phase transitions have no latent heat and are characterized by a change in symmetry. In addition to the conventional symmetric and antisymmetric states under permutations of bosons and fermions, mathematical group-representation theory allows for non-Abelian permutation symmetry. Such symmetry can be hidden in states with defined total spins of spinor gases, which can be formed in optical cavities. The present work shows that the symmetry reveals itself in spin-independent or coordinate-independent properties of these gases, namely as non-Abelian entropy in thermodynamic properties. In weakly interacting Fermi gases, two phases appear associated with fermionic and non-Abelian symmetry under permutations of particle states, respectively. The second-order transitions between the phases are characterized by discontinuities in specific heat. Unlike other phase transitions, the present ones are not caused by interactions and can appear even in ideal gases. Similar effects in Bose gases and strong interactions are discussed.

Anderson Transition of Cold Atoms with Synthetic Spin-Orbit Coupling in Two-Dimensional Speckle Potentials

Science.gov (United States)

Orso, Giuliano

2017-03-01

We investigate the metal-insulator transition occurring in two-dimensional (2D) systems of noninteracting atoms in the presence of artificial spin-orbit interactions and a spatially correlated disorder generated by laser speckles. Based on a high order discretization scheme, we calculate the precise position of the mobility edge and verify that the transition belongs to the symplectic universality class. We show that the mobility edge depends strongly on the mixing angle between Rashba and Dresselhaus spin-orbit couplings. For equal couplings a non-power-law divergence is found, signaling the crossing to the orthogonal class, where such a 2D transition is forbidden.

Spin-polarized scanning tunneling microscopy of magnetic nanostructures at the example of bcc-Co/Fe(110), Fe/Mo(110), and copper phthalocyanine/Fe(1110); Spinpolarisierte Rastertunnelmikroskopie magnetischer Nanostrukturen am Beispiel von bcc-Co/Fe(110), Fe/Mo(110) und Kupfer-Phthalocyanin/Fe(110)

Energy Technology Data Exchange (ETDEWEB)

Methfessel, Torsten

2010-12-09

This thesis provides an introduction into the technique of spin-polarized scanning tunnelling microscopy and spectroscopy as an experimental method for the investigation of magnetic nanostructures. Experimental results for the spin polarized electronic structure depending on the crystal structure of ultrathin Co layers, and depending on the direction of the magnetization for ultrathin Fe layers are presented. High-resolution measurements show the position-dependent spin polarization on a single copper-phthalocyanine molecule deposited on a ferromagnetic surface. Co was deposited by molecular beam epitaxy on the (110) surface of the bodycentered cubic metals Cr and Fe. In contrast to previous reports in the literature only two layers of Co can be stabilized in the body-centered cubic (bcc) structure. The bcc-Co films on the Fe(110) surface show no signs of epitaxial distortions. Thicker layers reconstruct into a closed-packed structure (hcp / fcc). The bcc structure increases the spin-polarization of Co to P=62 % in comparison to hcp-Co (P=45 %). The temperature-dependent spin-reorientation of ultrathin Fe/Mo(110) films was investigated by spin-polarized spectroscopy. A reorientation of the magnetic easy axis from the [110] direction along the surface normal to the in-plane [001] axis is observed at T (13.2{+-}0.5) K. This process can be identified as a discontinuous reorientation transition, revealing two simultaneous minima of the free energy in a certain temperature range. The electronic structure of mono- and double-layer Fe/Mo(110) shows a variation with the reorientation of the magnetic easy axis and with the direction of the magnetization. The investigation of the spin-polarized charge transport through a copper-phthalocyanine molecule on the Fe/Mo(110) surface provides an essential contribution to the understanding of spin-transport at the interface between metal and organic molecule. Due to the interaction with the surface of the metal the HOMO-LUMO energy

Mean-Field Studies of a Mixed Spin-3/2 and Spin-2 and a Mixed Spin-3/2 and Spin-5/2 Ising System with Different Anisotropies

International Nuclear Information System (INIS)

Wei Guozhu; Miao Hailing

2009-01-01

The magnetic properties of a mixed spin-3/2 and spin-2 and a mixed spin-3/2 and spin-5/2 Ising ferromagnetic system with different anisotropies are studied by means of mean-field theory (MFT). The dependence of the phase diagram on single-ion anisotropy strengths is studied too. In the mixed spin-3/2 and spin-2 Ising model, besides the second-order phase transition, the first order-disorder phase transition and the tricritical line are found. In the mixed spin-3/2 and spin-5/2 Ising model, there is no first-order transition and tricritical line. (condensed matter: electronic structure, electrical, magnetic, and optical properties)

k-asymmetric spin splitting at the interface between transition metal ferromagnets and heavy metals

KAUST Repository

Grytsiuk, Sergii

2016-05-23

We systematically investigate the spin-orbit coupling-induced band splitting originating from inversion symmetry breaking at the interface between a Co monolayer and 4d (Tc, Ru, Rh, Pd, and Ag) or 5d (Re, Os, Ir, Pt, and Au) transition metals. In spite of the complex band structure of these systems, the odd-in-k spin splitting of the bands displays striking similarities with the much simpler Rashba spin-orbit coupling picture. We establish a clear connection between the overall strength of the odd-in-k spin splitting of the bands and the charge transfer between the d orbitals at the interface. Furthermore, we show that the spin splitting of the Fermi surface scales with the induced orbital moment, weighted by the spin-orbit coupling.

k-asymmetric spin splitting at the interface between transition metal ferromagnets and heavy metals

KAUST Repository

Grytsyuk, Sergiy; Belabbes, Abderrezak; Haney, Paul M.; Lee, Hyun-Woo; Lee, Kyung-Jin; Stiles, M. D.; Schwingenschlö gl, Udo; Manchon, Aurelien

2016-01-01

We systematically investigate the spin-orbit coupling-induced band splitting originating from inversion symmetry breaking at the interface between a Co monolayer and 4d (Tc, Ru, Rh, Pd, and Ag) or 5d (Re, Os, Ir, Pt, and Au) transition metals. In spite of the complex band structure of these systems, the odd-in-k spin splitting of the bands displays striking similarities with the much simpler Rashba spin-orbit coupling picture. We establish a clear connection between the overall strength of the odd-in-k spin splitting of the bands and the charge transfer between the d orbitals at the interface. Furthermore, we show that the spin splitting of the Fermi surface scales with the induced orbital moment, weighted by the spin-orbit coupling.

Low to High Spin-State Transition Induced by Charge Ordering in Antiferromagnetic YBaCo2O5

International Nuclear Information System (INIS)

Vogt, T.; Woodward, P. M.; Karen, P.; Hunter, B. A.; Henning, P.; Moodenbaugh, A. R.

2000-01-01

The oxygen-deficient double perovskite YBaCo 2 O 5 , containing corner-linked CoO 5 square pyramids as principal building units, undergoes a paramagnetic to antiferromagnetic spin ordering at 330 K. This is accompanied by a tetragonal to orthorhombic distortion. Below 220 K orbital ordering and long-range Co 2+ /Co 3+ charge ordering occur as well as a change in the Co 2+ spin state from low to high spin. This transition is shown to be very sensitive to the oxygen content of the sample. To our knowledge this is the first observation of a spin-state transition induced by long-range orbital and charge ordering. (c) 2000 The American Physical Society

Spin-Polarization-Induced Preedge Transitions in the Sulfur K-Edge XAS Spectra of Open-Shell Transition-Metal Sulfates: Spectroscopic Validation of σ-Bond Electron Transfer.

Science.gov (United States)

Frank, Patrick; Szilagyi, Robert K; Gramlich, Volker; Hsu, Hua-Fen; Hedman, Britt; Hodgson, Keith O

2017-02-06

Sulfur K-edge X-ray absorption spectroscopy (XAS) spectra of the monodentate sulfate complexes [M II (itao)(SO 4 )(H 2 O) 0,1 ] (M = Co, Ni, Cu) and [Cu(Me 6 tren)(SO 4 )] exhibit well-defined preedge transitions at 2479.4, 2479.9, 2478.4, and 2477.7 eV, respectively, despite having no direct metal-sulfur bond, while the XAS preedge of [Zn(itao)(SO 4 )] is featureless. The sulfur K-edge XAS of [Cu(itao)(SO 4 )] but not of [Cu(Me 6 tren)(SO 4 )] uniquely exhibits a weak transition at 2472.1 eV, an extraordinary 8.7 eV below the first inflection of the rising K-edge. Preedge transitions also appear in the sulfur K-edge XAS of crystalline [M II (SO 4 )(H 2 O)] (M = Fe, Co, Ni, and Cu, but not Zn) and in sulfates of higher-valent early transition metals. Ground-state density functional theory (DFT) and time-dependent DFT (TDDFT) calculations show that charge transfer from coordinated sulfate to paramagnetic late transition metals produces spin polarization that differentially mixes the spin-up (α) and spin-down (β) spin orbitals of the sulfate ligand, inducing negative spin density at the sulfate sulfur. Ground-state DFT calculations show that sulfur 3p character then mixes into metal 4s and 4p valence orbitals and various combinations of ligand antibonding orbitals, producing measurable sulfur XAS transitions. TDDFT calculations confirm the presence of XAS preedge features 0.5-2 eV below the rising sulfur K-edge energy. The 2472.1 eV feature arises when orbitals at lower energy than the frontier occupied orbitals with S 3p character mix with the copper(II) electron hole. Transmission of spin polarization and thus of radical character through several bonds between the sulfur and electron hole provides a new mechanism for the counterintuitive appearance of preedge transitions in the XAS spectra of transition-metal oxoanion ligands in the absence of any direct metal-absorber bond. The 2472.1 eV transition is evidence for further radicalization from copper(II), which

Spin-glass-like transition in the majority-vote model with anticonformists

Science.gov (United States)

Krawiecki, Andrzej

2018-03-01

Majority-vote model on scale-free networks and random graphs is investigated in which a randomly chosen fraction p of agents (called anticonformists) follows an antiferromagnetic update rule, i.e., they assume, with probability governed by a parameter q (0 transition from a disordered (paramagnetic) state to a spin-glass-like state, characterized by a non-zero value of the spin-glass order parameter measuring the overlap of agents' opinions in two replicas of the system, and simultaneously by the magnetization close to zero. In the case of the model on scale-free networks the critical value of the parameter q weakly depends on the details of the degree distribution. As p is decreased, the critical value of q falls quickly to zero and only the disordered phase is observed. On the other hand, for p close to zero for decreasing q the usual ferromagnetic transition is observed.

Signatures of a quantum dynamical phase transition in a three-spin system in presence of a spin environment

International Nuclear Information System (INIS)

Alvarez, Gonzalo A.; Levstein, Patricia R.; Pastawski, Horacio M.

2007-01-01

We have observed an environmentally induced quantum dynamical phase transition in the dynamics of a two-spin experimental swapping gate [G.A. Alvarez, E.P. Danieli, P.R. Levstein, H.M. Pastawski, J. Chem. Phys. 124 (2006) 194507]. There, the exchange of the coupled states vertical bar ↑,↓> and vertical bar ↓,↑> gives an oscillation with a Rabi frequency b/ℎ (the spin-spin coupling). The interaction, ℎ/τ SE with a spin-bath degrades the oscillation with a characteristic decoherence time. We showed that the swapping regime is restricted only to bτ SE > or approx. ℎ. However, beyond a critical interaction with the environment the swapping freezes and the system enters to a Quantum Zeno dynamical phase where relaxation decreases as coupling with the environment increases. Here, we solve the quantum dynamics of a two-spin system coupled to a spin-bath within a Liouville-von Neumann quantum master equation and we compare the results with our previous work within the Keldysh formalism. Then, we extend the model to a three interacting spin system where only one is coupled to the environment. Beyond a critical interaction the two spins not coupled to the environment oscillate with the bare Rabi frequency and relax more slowly. This effect is more pronounced when the anisotropy of the system-environment (SE) interaction goes from a purely XY to an Ising interaction form

RECOILING SUPERMASSIVE BLACK HOLES IN SPIN-FLIP RADIO GALAXIES

International Nuclear Information System (INIS)

Liu, F. K.; Wang Dong; Chen Xian

2012-01-01

Numerical relativity simulations predict that coalescence of supermassive black hole (SMBH) binaries leads not only to a spin flip but also to a recoiling of the merger remnant SMBHs. In the literature, X-shaped radio sources are popularly suggested to be candidates for SMBH mergers with spin flip of jet-ejecting SMBHs. Here we investigate the spectral and spatial observational signatures of the recoiling SMBHs in radio sources undergoing black hole spin flip. Our results show that SMBHs in most spin-flip radio sources have mass ratio q ∼> 0.3 with a minimum possible value q min ≅ 0.05. For major mergers, the remnant SMBHs can get a kick velocity as high as 2100 km s –1 in the direction within an angle ∼< 40° relative to the spin axes of remnant SMBHs, implying that recoiling quasars are biased to be with high Doppler-shifted broad emission lines while recoiling radio galaxies are biased to large apparent spatial off-center displacements. We also calculate the distribution functions of line-of-sight velocity and apparent spatial off-center displacements for spin-flip radio sources with different apparent jet reorientation angles. Our results show that the larger the apparent jet reorientation angle is, the larger the Doppler-shifting recoiling velocity and apparent spatial off-center displacement will be. We investigate the effects of recoiling velocity on the dust torus in spin-flip radio sources and suggest that recoiling of SMBHs would lead to 'dust-poor' active galactic nuclei. Finally, we collect a sample of 19 X-shaped radio objects and for each object give the probability of detecting the predicted signatures of recoiling SMBH.

Orbital occupancy evolution across spin- and charge-ordering transitions in YBaFe2O5

Science.gov (United States)

Lindén, J.; Lindroos, F.; Karen, P.

2017-08-01

Thermal evolution of the Fe2+-Fe3+ valence mixing in YBaFe2O5 is investigated using Mössbauer spectroscopy. In this high-spin double-cell perovskite, the d6 and d5 Fe states differ by the single minority-spin electron which then controls all the spin- and charge-ordering transitions. Orbital occupancies can be extracted from the spectra in terms of the dxz , dz2 and either dx2-y2 (Main Article) or dxy (Supplement) populations of this electron upon conserving its angular momentum. At low temperatures, the minority-spin electrons fill up the ordered dxz orbitals of Fe2+, in agreement with the considerable orthorhombic distortion of the structure. Heating through the Verwey transition supplies 93% of the mixing entropy, at which point the predominantly mixing electron occupies mainly the dx2-y2 /dxy orbitals weakly bonding the two Fe atoms that face each other across the bases of their coordination pyramids. This might stabilize a weak coulombic checkerboard order suggested by McQueeney et alii in Phys. Rev. B 87(2013)045127. When the remaining 7% of entropy is supplied at a subsequent transition, the mixing electron couples the two Fe atoms predominantly via their dz2 orbitals. The valence mixing concerns more than 95% of the Fe atoms present in the crystalline solid; the rest is semi-quantitatively interpreted as domain walls and antiphase boundaries formed upon cooling through the Néel and Verwey-transition temperatures, respectively.

Structural phase transitions and weak ferromagnetism in La2-xNdxCuO4+δ

International Nuclear Information System (INIS)

Crawford, M.K.; Harlow, R.L.; McCarron, E.M.; Farneth, W.E.; Herron, N.; Chou, H.; Cox, D.E.

1993-01-01

When cooled, La 2-x Nd x CuO 4+δ undergoes structural transformations involving tilts of the CuO 6 octahedra which can be controlled by varying x and δ. Using synchrotron x-ray and neutron powder diffraction we observe that the transformation from Bmab to Pccn space-group symmetry is accompanied by a 90 degree copper spin reorientation in the basal plane. Furthermore, a second magnetic transition at lower temperatures yields weak ferromagnetism. These observations may have important implications for the suppression of superconductivity in the P4 2 /ncm phase of La 1.875 Ba 0.125 CuO 4

Quantum discord and quantum phase transition in spin chains

OpenAIRE

Dillenschneider, Raoul

2008-01-01

Quantum phase transitions of the transverse Ising and antiferromagnetic XXZ spin S=1/2 chains are studied using quantum discord. Quantum discord allows the measure of quantum correlations present in many-body quantum systems. It is shown that the amount of quantum correlations increases close to the critical points. The observations are in agreement with the information provided by the concurrence which measures the entanglement of the many-body system.

The light-induced spin transition of tetranuclear spin crossover complex [Fe4(CN)4(bpy)4(tpa)2](PF6)4

International Nuclear Information System (INIS)

Nishihara, T; Tanaka, K; Nihei, M; Oshio, H

2009-01-01

We report on the light induced spin transition in the tetranuclear spin crossover complex [Fe 4 (CN) 4 (bpy) 4 (tpa) 2 ](PF 6 ) 4 . The photo-conversion occurs at the specific site (Fe2) of four Fe II ions. The red light irradiation (1.79 eV) gives rise to full conversion of Fe2 into the high spin state from the low spin state. The green light irradiation (2.33 eV) can convert only the half of Fe2 into the high spin state, though the photo-conversion rate in the beginning is much higher than that with the red light. We present a simple model in which the photo-conversion kinetics is controlled by a large background absorption due to remaining three Fe II ions (Fe1, Fe3 and Fe4).

Spin-polarized spin excitation spectroscopy

International Nuclear Information System (INIS)

Loth, Sebastian; Lutz, Christopher P; Heinrich, Andreas J

2010-01-01

We report on the spin dependence of elastic and inelastic electron tunneling through transition metal atoms. Mn, Fe and Cu atoms were deposited onto a monolayer of Cu 2 N on Cu(100) and individually addressed with the probe tip of a scanning tunneling microscope. Electrons tunneling between the tip and the substrate exchange energy and spin angular momentum with the surface-bound magnetic atoms. The conservation of energy during the tunneling process results in a distinct onset threshold voltage above which the tunneling electrons create spin excitations in the Mn and Fe atoms. Here we show that the additional conservation of spin angular momentum leads to different cross-sections for spin excitations depending on the relative alignment of the surface spin and the spin of the tunneling electron. For this purpose, we developed a technique for measuring the same local spin with a spin-polarized and a non-spin-polarized tip by exchanging the last apex atom of the probe tip between different transition metal atoms. We derive a quantitative model describing the observed excitation cross-sections on the basis of an exchange scattering process.

Photoinduced Coherent Spin Fluctuation in Primary Dynamics of Insulator to Metal Transition in Perovskite Cobalt Oxide

Directory of Open Access Journals (Sweden)

Arima T.

2013-03-01

Full Text Available Coherent spin fluctuation was detected in the photoinduced Mott insulator-metal transition in perovskite cobalt oxide by using 3 optical-cycle infrared pulse. Such coherent spin fluctuation is driven by the perovskite distortion changing orbital gap.

Spin transfer in reactions between heavy ions

International Nuclear Information System (INIS)

Dong Pil Min.

1980-06-01

The model presented affords a better understanding of the manner in which the orbital angular moment can be converted into an intrinsic spin in the collision between two heavy ions. After referring to the vector fields and the collective energy of a spheroidal nucleus, the calculation of the exchange of nucleons is described and the dissipation function is constructed. The spin transfer and the reorientation of the spin during the reaction are then examined (effect of friction and vibration). The estimated calculations are compared with the results of the 63 Cu+ 197 Au and 86 Kr+ 209 Bi experiments. The sensitivity of the calculation to the parameters of the model is discussed (nuclear potential, vibrational inertial parameter) [fr

Mixed-order phase transition in a minimal, diffusion-based spin model.

Science.gov (United States)

Fronczak, Agata; Fronczak, Piotr

2016-07-01

In this paper we exactly solve, within the grand canonical ensemble, a minimal spin model with the hybrid phase transition. We call the model diffusion based because its Hamiltonian can be recovered from a simple dynamic procedure, which can be seen as an equilibrium statistical mechanics representation of a biased random walk. We outline the derivation of the phase diagram of the model, in which the triple point has the hallmarks of the hybrid transition: discontinuity in the average magnetization and algebraically diverging susceptibilities. At this point, two second-order transition curves meet in equilibrium with the first-order curve, resulting in a prototypical mixed-order behavior.

Disentanglement of two qubits coupled to an XY spin chain: Role of quantum phase transition

International Nuclear Information System (INIS)

Yuan Zigang; Li Shushen; Zhang Ping

2007-01-01

We study the disentanglement evolution of two spin qubits which interact with a general XY spin-chain environment. The dynamical process of the disentanglement is numerically and analytically investigated in the vicinity of a quantum phase transition (QPT) of the spin chain in both weak and strong coupling cases. We find that the disentanglement of the two spin qubits may be greatly enhanced by the quantum critical behavior of the environmental spin chain. We give a detailed analysis to facilitate the understanding of the QPT-enhanced decaying behavior of the coherence factor. Furthermore, the scaling behavior in the disentanglement dynamics is also revealed and analyzed

Reorientational dynamics in molecular liquids as revealed by dynamic light scattering: from boiling point to glass transition temperature.

Science.gov (United States)

Schmidtke, B; Petzold, N; Kahlau, R; Rössler, E A

2013-08-28

We determine the reorientational correlation time τ of a series of molecular liquids by performing depolarized light scattering experiments (double monochromator, Fabry-Perot interferometry, and photon correlation spectroscopy). Correlation times in the range 10(-12) s-100 s are compiled, i.e., the full temperature interval between the boiling point and the glass transition temperature T(g) is covered. We focus on low-T(g) liquids for which the high-temperature limit τ ≅ 10(-12) s is easily accessed by standard spectroscopic equipment (up to 440 K). Regarding the temperature dependence three interpolation formulae of τ(T) with three parameters each are tested: (i) Vogel-Fulcher-Tammann equation, (ii) the approach recently discussed by Mauro et al. [Proc. Natl. Acad. Sci. U.S.A. 106, 19780 (2009)], and (iii) our approach decomposing the activation energy E(T) in a constant high temperature value E∞ and a "cooperative part" E(coop)(T) depending exponentially on temperature [Schmidtke et al., Phys. Rev. E 86, 041507 (2012)]. On the basis of the present data, approaches (i) and (ii) are insufficient as they do not provide the correct crossover to the high-temperature Arrhenius law clearly identified in the experimental data while approach (iii) reproduces the salient features of τ(T). It allows to discuss the temperature dependence of the liquid's dynamics in terms of a E(coop)(T)/E∞ vs. T/E∞ plot and suggests that E∞ controls the energy scale of the glass transition phenomenon.

Effect of hydrostatic pressure on magnetic phase transitions and magnetization in gadolinium monocrystal

International Nuclear Information System (INIS)

Nikitin, S.A.; Bezdushnyj, R.V.

1989-01-01

Effect of hydrostatic pressure on magnetization in gadolinium monocrystal (Δσ-effect) was investigated. Dependences of spesific magnetization, Δσ-effect and bulk magnetostriction of gadolinium monocrystal on temperatures were studied. Results of conducted investigation have shown that in gadolinium the change of specific magnetization under the hydrostatic pressure effect is caused in general case by three effects: a)change of spontaneous magnetization under the effect of hydrostatic pressure; b)change of magnetization within technical magnetization range due to the effect of hydrostatic pressure on magnetic anisotropy constants; c)change of magnetization due to the effect of hydrostatic pressure on temperature of spin-reoriented transition

Effects of the substitution of iron for cobalt on the crystal and magnetic properties of PrCo4-xFexM (M=Al and Ga)

International Nuclear Information System (INIS)

Zlotea, C.; Isnard, O.

2003-01-01

We report on the structural and magnetic properties of PrCo 4-x Fe x M where x=0-4 and M=Al and Ga. The iron solubility limit in these phases is determined by means of X-ray diffraction and scanning electron microscopy. Our study confirms that single phase samples crystallizing in the CaCu 5 -type structure are stabilized for x 5 structure but with a slight preference for the 3g site. The saturation magnetization and the Curie temperature increase upon the iron substitution. The PrCo 4-x Fe x M compounds present spin reorientation transitions, whatever the substituting M and the Fe content. The substitution of iron for cobalt induces a significant increase of the spin reorientation temperature. Neutron and X-ray powder diffraction experiments as well as magnetic measurements are combined in order to clarify the effects of the presence of iron on the magnetocrystalline anisotropy and the spin reorientation transition. Finally, the magnetic phase diagrams of PrCo 4-x Fe x M (M=Al and Ga) have been determined in the whole ordered temperature range

Isotope enrichment by electron spin resonance transitions of the intermediate radical pair

International Nuclear Information System (INIS)

Okazaki, M.; Shiga, T.; Sakata, S.; Konaka, R.; Toriyama, K.

1988-01-01

Microwave effects on the spin adduct yield were observed in the photoreduction of menadione in micellar solutions with ordinary sodium dodecyl sulfate (SDS), deuterium-labeled SDS, and a mixture of them. A large isotope effect was found in the microwave modulation of the spin adduct yield, which is due to the ESR transitions of the transient radical pair in the reaction. It is demonstrated for the first time that the microwave field can be used to enrich one of the isotopes which coexist in the system

Evidence for reentrant spin glass behavior in transition metal substituted Co-Ga alloys near critical concentration

Science.gov (United States)

Yasin, Sk. Mohammad; Srinivas, V.; Kasiviswanathan, S.; Vagadia, Megha; Nigam, A. K.

2018-04-01

In the present study magnetic and electrical transport properties of transition metal substituted Co-Ga alloys (near critical cobalt concentration) have been investigated. Analysis of temperature and field dependence of dc magnetization and ac susceptibility (ACS) data suggests an evidence of reentrant spin glass (RSG) phase in Co55.5TM3Ga41.5 (TM = Co, Cr, Fe, Cu). The magnetic transition temperatures (TC and Tf) are found to depend on the nature of TM element substitution with the exchange coupling strength Co-Fe > Co-Co > Co-Cu > Co-Cr. From magnetization dynamics precise transition temperatures for the glassy phases are estimated. It is found that characteristic relaxation times are higher than that of spin glasses with minimal spin-cluster formation. The RSG behavior has been further supported by the temperature dependence of magnetotransport studies. From the magnetic field and substitution effects it has been established that the magnetic and electrical transport properties are correlated in this system.

Signatures for isoscalar spin transitions excited in (d, d,) reactions

International Nuclear Information System (INIS)

Morlet, M.; Willis, A.; Van de Wiele, J.; Marty, N.; Guillot, J.; Langevin-Joliot, H.; Bimbot, L.; Rosier, L.; Djalali, C.; Duchazeaubeneix, J.C.

1990-01-01

Three different signatures for isoscalar spin transitions in nuclei have been tested in the 12 C(d, d , ) 12 C reaction at 400 MeV. These signatures have values of close to zero for the natural parity states, and values ranging from 0.22 to 0.50 for the ΔS=1 ΔT=0, 12.7 MeV state

Quantum phase transitions in effective spin-ladder models for graphene zigzag nanoribbons

Science.gov (United States)

Koop, Cornelie; Wessel, Stefan

2017-10-01

We examine the magnetic correlations in quantum spin models that were derived recently as effective low-energy theories for electronic correlation effects on the edge states of graphene nanoribbons. For this purpose, we employ quantum Monte Carlo simulations to access the large-distance properties, accounting for quantum fluctuations beyond mean-field-theory approaches to edge magnetism. For certain chiral nanoribbons, antiferromagnetic interedge couplings were previously found to induce a gapped quantum disordered ground state of the effective spin model. We find that the extended nature of the intraedge couplings in the effective spin model for zigzag nanoribbons leads to a quantum phase transition at a large, finite value of the interedge coupling. This quantum critical point separates the quantum disordered region from a gapless phase of stable edge magnetism at weak intraedge coupling, which includes the ground states of spin-ladder models for wide zigzag nanoribbons. To study the quantum critical behavior, the effective spin model can be related to a model of two antiferromagnetically coupled Haldane-Shastry spin-half chains with long-ranged ferromagnetic intrachain couplings. The results for the critical exponents are compared also to several recent renormalization-group calculations for related long-ranged interacting quantum systems.

Magnetovolume effects and magnetic transitions in the invar systems Fe65Ni35 and Er2Fe14B at high hydrostatic pressure

International Nuclear Information System (INIS)

Sidorov, V.A.; Khvostantsev, L.G.

1994-01-01

The relative volume change and the initial ac-susceptibility have been measured for Fe 65 Ni 35 and Er 2 Fe 14 B under hydrostatic pressure up to 8.5 GPa at room temperature. The bulk modulus of Fe 65 Ni 35 begins to rise and the susceptibility begins to drop at 3.5-4 GPa, indicating the continuous disappearance of ferromagnetism at high pressure. The transition from ferromagnetic to paramagnetic state in Er 2 Fe 14 B at 5.7 GPa is more abrupt and the giant (order of magnitude) softening of the bulk modulus is observed before this transition. The spin reorientation (SR) transition in Er 2 Fe 14 B shifts under pressure to lower temperatures (dT SR /dP = -19 K/GPa). (orig.)

Dynamic-angle spinning and double rotation of quadrupolar nuclei

International Nuclear Information System (INIS)

Mueller, K.T.; California Univ., Berkeley, CA

1991-07-01

Nuclear magnetic resonance (NMR) spectroscopy of quadrupolar nuclei is complicated by the coupling of the electric quadrupole moment of the nucleus to local variations in the electric field. The quadrupolar interaction is a useful source of information about local molecular structure in solids, but it tends to broaden resonance lines causing crowding and overlap in NMR spectra. Magic- angle spinning, which is routinely used to produce high resolution spectra of spin-1/2 nuclei like carbon-13 and silicon-29, is incapable of fully narrowing resonances from quadrupolar nuclei when anisotropic second-order quadrupolar interactions are present. Two new sample-spinning techniques are introduced here that completely average the second-order quadrupolar coupling. Narrow resonance lines are obtained and individual resonances from distinct nuclear sites are identified. In dynamic-angle spinning (DAS) a rotor containing a powdered sample is reoriented between discrete angles with respect to high magnetic field. Evolution under anisotropic interactions at the different angles cancels, leaving only the isotropic evolution of the spin system. In the second technique, double rotation (DOR), a small rotor spins within a larger rotor so that the sample traces out a complicated trajectory in space. The relative orientation of the rotors and the orientation of the larger rotor within the magnetic field are selected to average both first- and second-order anisotropic broadening. The theory of quadrupolar interactions, coherent averaging theory, and motional narrowing by sample reorientation are reviewed with emphasis on the chemical shift anisotropy and second-order quadrupolar interactions experienced by half-odd integer spin quadrupolar nuclei. The DAS and DOR techniques are introduced and illustrated with application to common quadrupolar systems such as sodium-23 and oxygen-17 nuclei in solids

Dynamic-angle spinning and double rotation of quadrupolar nuclei

Energy Technology Data Exchange (ETDEWEB)

Mueller, K.T. (Lawrence Berkeley Lab., CA (United States) California Univ., Berkeley, CA (United States). Dept. of Chemistry)

1991-07-01

Nuclear magnetic resonance (NMR) spectroscopy of quadrupolar nuclei is complicated by the coupling of the electric quadrupole moment of the nucleus to local variations in the electric field. The quadrupolar interaction is a useful source of information about local molecular structure in solids, but it tends to broaden resonance lines causing crowding and overlap in NMR spectra. Magic- angle spinning, which is routinely used to produce high resolution spectra of spin-{1/2} nuclei like carbon-13 and silicon-29, is incapable of fully narrowing resonances from quadrupolar nuclei when anisotropic second-order quadrupolar interactions are present. Two new sample-spinning techniques are introduced here that completely average the second-order quadrupolar coupling. Narrow resonance lines are obtained and individual resonances from distinct nuclear sites are identified. In dynamic-angle spinning (DAS) a rotor containing a powdered sample is reoriented between discrete angles with respect to high magnetic field. Evolution under anisotropic interactions at the different angles cancels, leaving only the isotropic evolution of the spin system. In the second technique, double rotation (DOR), a small rotor spins within a larger rotor so that the sample traces out a complicated trajectory in space. The relative orientation of the rotors and the orientation of the larger rotor within the magnetic field are selected to average both first- and second-order anisotropic broadening. The theory of quadrupolar interactions, coherent averaging theory, and motional narrowing by sample reorientation are reviewed with emphasis on the chemical shift anisotropy and second-order quadrupolar interactions experienced by half-odd integer spin quadrupolar nuclei. The DAS and DOR techniques are introduced and illustrated with application to common quadrupolar systems such as sodium-23 and oxygen-17 nuclei in solids.

Superconductor to spin-density-wave transition in quasi-one-dimensional metals with repulsive anisotropic interaction

International Nuclear Information System (INIS)

Rozhkov, A.V.

2007-01-01

A mechanism for superconductivity in a quasi-one-dimensional system with repulsive Ising-anisotropic interaction is studied. The Ising anisotropy opens the gap Δ s in the spin sector of the model. This gap allows the triplet superconductivity and the spin-density wave as the only broken symmetry phases. These phases are separated by the first order transition. The transport properties of the system are investigated in different parts of the phase diagram. The calculation of DC conductivity σ(T) in the high-temperature phase shows that the function σ(T) cannot be used as an indicator of a superconducting ground state: even if σ(T) is a decreasing function at high temperature, yet, the ground state may be insulating spin-density wave; the opposite is also true. The calculation of the spin dynamical structure factor S zz (q, ω) demonstrates that it is affected by the superconducting phase transition in a qualitative fashion: below T c the structure factor develops a gap with a coherent excitation inside this gap

Self-Reorientation Following Colorectal Cancer Treatment - A Grounded Theory Study.

Science.gov (United States)

Johansson, Ann-Caroline B; Axelsson, Malin; Berndtsson, Ina; Brink, Eva

2015-01-01

After colorectal cancer (CRC) treatment, people reorganize life in ways that are consistent with their understanding of the illness and their expectations for recovery. Incapacities and abilities that have been lost can initiate a need to reorient the self. To the best of our knowledge, no studies have explicitly focused on the concept of self-reorientation after CRC treatment. The aim of the present study was therefore to explore self-reorientation in the early recovery phase after CRC surgery. Grounded theory analysis was undertaken, using the method presented by Charmaz. The present results explained self-reorientation as the individual attempting to achieve congruence in self-perception. A congruent self-perception meant bringing together the perceived self and the self that was mirrored in the near environs. The results showed that societal beliefs and personal explanations are essential elements of self-reorientation, and that it is therefore important to make them visible.

Lattice architecture effect on the cooperativity of spin transition coordination polymers

Energy Technology Data Exchange (ETDEWEB)

Chiruta, Daniel [Faculty of Electrical Engineering and Computer Science and Advanced Materials and Nanotechnology Laboratory (AMNOL), Ştefan cel Mare University, Suceava 720229 (Romania); GEMaC, Université de Versailles Saint-Quentin-en-Yvelines, CNRS-UVSQ (UMR 8635), 78035 Versailles Cedex (France); LISV, Université de Versailles Saint-Quentin-en-Yvelines, 78140 Velizy (France); Jureschi, Catalin-Maricel; Rotaru, Aurelian, E-mail: jorge.linares@uvsq.fr, E-mail: rotaru@eed.usv.ro [Faculty of Electrical Engineering and Computer Science and Advanced Materials and Nanotechnology Laboratory (AMNOL), Ştefan cel Mare University, Suceava 720229 (Romania); Linares, Jorge, E-mail: jorge.linares@uvsq.fr, E-mail: rotaru@eed.usv.ro [GEMaC, Université de Versailles Saint-Quentin-en-Yvelines, CNRS-UVSQ (UMR 8635), 78035 Versailles Cedex (France); Garcia, Yann [Institute of Condensed Matter and Nanosciences, Molecules, Solids and Reactivity (IMCN/MOST), Université Catholique de Louvain, Place L. Pasteur, 1, 1348 Louvain-la-Neuve (Belgium)

2014-02-07

We have investigated in the framework of the Ising-like model, by means of Monte Carlo Metropolis method with open boundary condition, the architecture effect on the cooperativity of spin transition coordination polymers. We have analyzed the influence of several physical parameters (size, pressure, and edge effects) on different lattice architectures which were in good agreement with reported experimental data. We show that the cooperativity of a spin crossover system, characterized by the same number of molecules and the same short- and long-range interaction parameters, is progressively enhanced when going from a 1D chain to a 1D ladder type lattice and to a 2D square lattice.

Study of transitional Erbium nuclei (N=86) at very high spin. Highlight of dipolar transitions and medium livetimes in the continuum

International Nuclear Information System (INIS)

Bogaert, G.

1984-01-01

Average lifetimes and multipolarities of unresolved transitions deexciting very high spin states of the light Rare Earth nuclei (N approximately 86) have been determined by a measure of Doppler shift attenuation and their anisotropy. The spin selection is provided by the total energy spectrometer technique; great care was taken of the existence of many long lived isomeric states in the studied nuclei. The N approximately 86 nuclei have been formed in the 84 Kr(340 MeV) + 74 Ge → 158 Er* reactions using the 84 Kr beam of the Orsay ALICE facilities and targets of 74 Ge built at the PARIS Isotope separator of the CSNSM. NaI γ spectra have been thoroughly cleared of the discrete lines contribution through a carefull subtraction procedure synthetising NaI spectra from the Ge ones. At very high spin the continuum γ rays feed two well separated bumps with Esub(γ) approximately .65 MeV and Esub(γ) approximately 1.3 MeV. The 1.3 MeV transitions appear at I > 30 h and their energy does not vary with the increasing spin like expected in the rotational case of the well deformed nuclei; they are strongly collectively enhanced with B(E2) > 130 W.u. Below 1 MeV the anisotropy of transitions is R approximately 0.7, indicating their stretched dipole nature. Recent calculations of nuclear shape deformation (following Strutinsky shell correction method) reproduce the two bumps shape of the experimental spectra and the origin of the excitation is explained in terms of nuclear vibration (γ-vibration, wobbling motion) [fr

A Study of the Spin-State Transition and Phase Transformation in [Fe(bpp)(2)][CF(3)SO(3)](2).H(2)O and [Fe(bpp)(2)][BF(4)](2) Using Mn(2+) Electron Spin Resonance.

Science.gov (United States)

Sung, Raymond C. W.; McGarvey, Bruce R.

1999-08-09

X-band ESR powder studies have been done on the spin transition in Mn(2+)-doped [Fe(bpp)(2)][CF(3)SO(3)](2).H(2)O and [Fe(bpp)(2)][BF(4)](2) (bpp = 2,6-bis(pyrazol-3-yl) pyridine). The change in D value of Mn(2+) during the thermally induced high-spin (HS) low-spin (LS) transition shows that the spin transition is accompanied by a phase transformation involving a domain mechanism. Irradiation experiments at 77 K have shown that a LS --> HS spin change occurs without a change in the crystalline phase. The rate of the change from the HS phase to the LS phase in the vicinity of 100 K has been measured and is found to be the same as that measured for the corresponding spin change obtained from Mössbauer spectroscopy and magnetic susceptibility studies.

Role of nuclear penetration effects in spin assignments. [J, transitions, internal conversion

Energy Technology Data Exchange (ETDEWEB)

Sahota, H S [Punjabi Univ., Patiala (India). Dept. of Physics

1976-04-01

Nuclear penetrations have been found to affect the internal conversion process of the retarded magnetic dipole transitions. In all cases where the penetration coefficient has been found to be essentially different from unity the transition is 1-forbidden. This criterian has been applied to the case of 191 keV transition in /sup 197/Au where the spin of the 268 keV level could not be deduced uniquely by any of the existing methods. The result is that the 199 keV transition has a dynamic contribution to its internal conversion process with the penetration coefficient lambda = 5.5 +- 0.9. To illustrate the applicability of the criterian further two more cases namely that of the 92 keV transition in /sup 131/Cs and 182 keV transition in /sup 129/Cs are also included.

Phase Transition in the Density of States of Quantum Spin Glasses

Energy Technology Data Exchange (ETDEWEB)

Erdős, László, E-mail: lerdos@ist.ac.at [IST Austria (Austria); Schröder, Dominik, E-mail: schroeder.dominik@gmail.com [Ludwig-Maximilians-Universität München (Germany)

2014-12-15

We prove that the empirical density of states of quantum spin glasses on arbitrary graphs converges to a normal distribution as long as the maximal degree is negligible compared with the total number of edges. This extends the recent results of Keating et al. (2014) that were proved for graphs with bounded chromatic number and with symmetric coupling distribution. Furthermore, we generalise the result to arbitrary hypergraphs. We test the optimality of our condition on the maximal degree for p-uniform hypergraphs that correspond to p-spin glass Hamiltonians acting on n distinguishable spin- 1/2 particles. At the critical threshold p = n{sup 1/2} we find a sharp classical-quantum phase transition between the normal distribution and the Wigner semicircle law. The former is characteristic to classical systems with commuting variables, while the latter is a signature of noncommutative random matrix theory.

The ferromagnetic-spin glass transition in PdMn alloys: symmetry breaking of ferromagnetism and spin glass studied by a multicanonical method.

Science.gov (United States)

Kato, Tomohiko; Saita, Takahiro

2011-03-16

The magnetism of Pd(1-x)Mn(x) is investigated theoretically. A localized spin model for Mn spins that interact with short-range antiferromagnetic interactions and long-range ferromagnetic interactions via itinerant d electrons is set up, with no adjustable parameters. A multicanonical Monte Carlo simulation, combined with a procedure of symmetry breaking, is employed to discriminate between the ferromagnetic and spin glass orders. The transition temperature and the low-temperature phase are determined from the temperature variation of the specific heat and the probability distributions of the ferromagnetic order parameter and the spin glass order parameter at different concentrations. The calculation results reveal that only the ferromagnetic phase exists at x glass phase exists at x > 0.04, and that the two phases coexist at intermediate concentrations. This result agrees semi-quantitatively with experimental results.

Unifying Exchange Sensitivity in Transition-Metal Spin-State Ordering and Catalysis through Bond Valence Metrics.

Science.gov (United States)

Gani, Terry Z H; Kulik, Heather J

2017-11-14

Accurate predictions of spin-state ordering, reaction energetics, and barrier heights are critical for the computational discovery of open-shell transition-metal (TM) catalysts. Semilocal approximations in density functional theory, such as the generalized gradient approximation (GGA), suffer from delocalization error that causes them to overstabilize strongly bonded states. Descriptions of energetics and bonding are often improved by introducing a fraction of exact exchange (e.g., erroneous low-spin GGA ground states are instead correctly predicted as high-spin with a hybrid functional). The degree of spin-splitting sensitivity to exchange can be understood based on the chemical composition of the complex, but the effect of exchange on reaction energetics within a single spin state is less well-established. Across a number of model iron complexes, we observe strong exchange sensitivities of reaction barriers and energies that are of the same magnitude as those for spin splitting energies. We rationalize trends in both reaction and spin energetics by introducing a measure of delocalization, the bond valence of the metal-ligand bonds in each complex. The bond valence thus represents a simple-to-compute property that unifies understanding of exchange sensitivity for catalytic properties and spin-state ordering in TM complexes. Close agreement of the resulting per-metal-organic-bond sensitivity estimates, together with failure of alternative descriptors demonstrates the utility of the bond valence as a robust descriptor of how differences in metal-ligand delocalization produce differing relative energetics with exchange tuning. Our unified description explains the overall effect of exact exchange tuning on the paradigmatic two-state FeO + /CH 4 reaction that combines challenges of spin-state and reactivity predictions. This new descriptor-sensitivity relationship provides a path to quantifying how predictions in transition-metal complex screening are sensitive to the

Pressure variation of Rashba spin splitting toward topological transition in the polar semiconductor BiTeI

Science.gov (United States)

Ideue, T.; Checkelsky, J. G.; Bahramy, M. S.; Murakawa, H.; Kaneko, Y.; Nagaosa, N.; Tokura, Y.

2014-10-01

BiTeI is a polar semiconductor with gigantic Rashba spin-split bands in bulk. We have investigated the effect of pressure on the electronic structure of this material via magnetotransport. Periods of Shubunikov-de Haas (SdH) oscillations originating from the spin-split outer Fermi surface and inner Fermi surface show disparate responses to pressure, while the carrier number derived from the Hall effect is unchanged with pressure. The associated parameters which characterize the spin-split band structure are strongly dependent on pressure, reflecting the pressure-induced band deformation. We find the SdH oscillations and transport response are consistent with the theoretically proposed pressure-induced band deformation leading to a topological phase transition. Our analysis suggests the critical pressure for the quantum phase transition near Pc=3.5 GPa.

Double exchange model on triangular lattice: Non-coplanar spin configuration and phase transition near quarter filling

Energy Technology Data Exchange (ETDEWEB)

Zhang, G.P., E-mail: bugubird_zhang@hotmail.com [Department of Physics, Renmin University of China, Beijing 100872 (China); Zhang, Jian [3M Company, 3M Corporate Headquarters, 3M Center, St. Paul, MN 55144-1000 (United States); Zhang, Qi-Li [Data Center for High Energy Density Physics, Institute of Applied Physics and Computational Mathematics, Beijing 100094 (China); Zhou, Jiang-Tao [College of Optoelectronic Engineering, Shenzhen University, Shenzhen 518060 (China); Shangguan, M.H. [Department of Physics, Renmin University of China, Beijing 100872 (China)

2013-05-15

Unconventional anomalous Hall effect in frustrated pyrochlore oxides is originated from spin chirality of non-coplanar localized spins, which can also be induced by the competition between ferromagnetic (FM) double exchange interaction J{sub H} and antiferromagnetic superexchange interaction J{sub AF}. Here truncated polynomial expansion method and Monte Carlo simulation are adopted to investigate the above model on two-dimensional triangular lattice. We discuss the influence of the range of FM-type spin–spin correlation and strong electron–spin correlation on the truncation error of spin–spin correlation near quarter filling. Two peaks of the probability distribution of spin–spin correlation in non-coplanar spin configuration clearly show that non-coplanar spin configuration is an intermediate phase between FM and 120° spin phase. Near quarter filling, there is a phase transition from FM into non-coplanar and further into 120° spin phase when J{sub AF} continually increases. Finally the effect of temperature on the magnetic structure is discussed.

Raman study of molecular motions in relation to phase transitions in [Ni(NH3)6](NO3)2

International Nuclear Information System (INIS)

Janik, J.M.; Pick, R.M.; Le Postollec, M.

1987-01-01

A Raman band at 710 cm -1 has been used for the study of the NO 3 - ions reorientation and of the phase transitions in [Ni(NH 3 ) 6 ](NO 3 ) 2 . The strong temperature dependence of the width of this band in phase 1 gives evidence for the NO 3 - reorientations in this phase. The reorientations stop in phase 2. The same band was used for studying the phase 2/phase 3 transition. The large thermal hysteresis of this transition has ben confirmed. 16 refs., 4 figs. (author)

Sexual reorientation therapy: an orthodox perspective.

Science.gov (United States)

Carlton, Clark

2004-01-01

This article evaluates the phenomenon of sexual reorientation therapy from the standpoint of Orthodox Christian theology. It is argued that homosexual desire is the product of the fall of mankind and cannot be considered "normal." At the same time, however, reorientation therapies, whether secular or Christian, are inherently reductionistic and fail to address the underlying spiritual pathologies involved in homosexual desire (or any other deep-seated passion). The purpose of therapeia in the Orthodox Church is the psycho-somatic transfiguration of the whole person into the image of Christ, not merely the cessation of homosexual activity or the "reidentification" of one's "lifestyle."

Vibrations and reorientations of H2O molecules in [Sr(H2O)6]Cl2 studied by Raman light scattering, incoherent inelastic neutron scattering and proton magnetic resonance.

Science.gov (United States)

Hetmańczyk, Joanna; Hetmańczyk, Lukasz; Migdał-Mikuli, Anna; Mikuli, Edward; Florek-Wojciechowska, Małgorzata; Harańczyk, Hubert

2014-04-24

Vibrational-reorientational dynamics of H2O ligands in the high- and low-temperature phases of [Sr(H2O)6]Cl2 was investigated by Raman Spectroscopy (RS), proton magnetic resonance ((1)H NMR), quasielastic and inelastic incoherent Neutron Scattering (QENS and IINS) methods. Neutron powder diffraction (NPD) measurements, performed simultaneously with QENS, did not indicated a change of the crystal structure at the phase transition (detected earlier by differential scanning calorimetry (DSC) at TC(h)=252.9 K (on heating) and at TC(c)=226.5K (on cooling)). Temperature dependence of the full-width at half-maximum (FWHM) of νs(OH) band at ca. 3248 cm(-1) in the RS spectra indicated small discontinuity in the vicinity of phase transition temperature, what suggests that the observed phase transition may be associated with a change of the H2O reorientational dynamics. However, an activation energy value (Ea) for the reorientational motions of H2O ligands in both phases is nearly the same and equals to ca. 8 kJ mol(-1). The QENS peaks, registered for low temperature phase do not show any broadening. However, in the high temperature phase a small QENS broadening is clearly visible, what implies that the reorientational dynamics of H2O ligands undergoes a change at the phase transition. (1)H NMR line is a superposition of two powder Pake doublets, differentiated by a dipolar broadening, suggesting that there are two types of the water molecules in the crystal lattice of [Sr(H2O)6]Cl2 which are structurally not equivalent average distances between the interacting protons are: 1.39 and 1.18 Å. However, their reorientational dynamics is very similar (τc=3.3⋅10(-10) s). Activation energies for the reorientational motion of these both kinds of H2O ligands have nearly the same values in an experimental error limit: and equal to ca. 40 kJ mole(-1). The phase transition is not seen in the (1)H NMR spectra temperature dependencies. Infrared (IR), Raman (RS) and inelastic

First-order phase transition in the quantum spin glass at T=0

Energy Technology Data Exchange (ETDEWEB)

Viana, J. Roberto; Nogueira, Yamilles; Sousa, J. Ricardo de

2003-05-26

The van Hemmen model with transverse and random longitudinal field is studied to analyze the tricritical behavior in the quantum Ising spin glass at T=0. The free energy and order parameter are calculated for two types of probability distributions: Gaussian and bimodal. We obtain the phase diagram in the {omega}-H plane, where {omega} and H are the transverse and random longitudinal fields, respectively. For the case of Gaussian distribution the phase transition is of second order, while the bimodal distribution we observe second-order transition for high-transverse field and first-order transition for small transverse field, with a tricritical point in the phase diagram.

First-order phase transition in the quantum spin glass at T=0

International Nuclear Information System (INIS)

Viana, J. Roberto; Nogueira, Yamilles; Sousa, J. Ricardo de

2003-01-01

The van Hemmen model with transverse and random longitudinal field is studied to analyze the tricritical behavior in the quantum Ising spin glass at T=0. The free energy and order parameter are calculated for two types of probability distributions: Gaussian and bimodal. We obtain the phase diagram in the Ω-H plane, where Ω and H are the transverse and random longitudinal fields, respectively. For the case of Gaussian distribution the phase transition is of second order, while the bimodal distribution we observe second-order transition for high-transverse field and first-order transition for small transverse field, with a tricritical point in the phase diagram

Direct measurement of the low temperature spin state transitions in La1-xSrxCoO3 (0.05 < x < 0.3)

Science.gov (United States)

Gulec, A.; Klie, R. F.

2014-12-01

Sr-doped LaCoO3 has a complex magnetic phase diagram, which is believed to be directly correlated to changes in the crystal structure and ordering of the Co3+ spin states. In this work, we study the low temperature Co3+-ion spin state transitions in Sr-doped LaCoO3 around the critical doping concentration where a metal to insulator transition has been observed using electron energy-loss spectroscopy of the O K-edge combined with the Co L-edge fine structure. We measure the local spin state of the Co3+-ions and we demonstrate that the Co3+ spin-state transition only occurs in La0.95Sr0.05CoO3 single-crystal materials in the temperature range accessible by LN2 in-situ cooling, while no structural symmetry change is observed. The presence of this low-temperature spin-state transition in La1-xSrxCoO3 (x < 0.17) has been proposed as the origin of the percolative magnetic ordering in doped LaCoO3.

Generation of a third harmonic due to spin-flip transitions in non-symmetric heterostructures

CERN Document Server

Korovin, A V

2003-01-01

The third-order non-linear response due to spin-flip transitions of electrons in asymmetric narrow-gap quantum wells with a spin-split energy spectrum is calculated. The resonant spectral dependences and the gate-voltage dependences of the third-order susceptibility are obtained. The efficiency of up-conversion of the microwave pumping into submillimetre radiation in the multi-well structure is estimated and the dependences on the incidence angle and on the polarization of pumping are presented.

Effective Parenting and Socialization for Value Re-Orientation in ...

African Journals Online (AJOL)

The paper discusses the meaning/concept and nature of parenting, effective parenting, some problems of parenting in Nigeria, socialization as a medium of value inculcation and value reorientation. The paper believes that value reorientation in Nigeria is a feasible project that can only be attained through the enforcement ...

Vibration dependence of the tensor spin-spin and scalar spin-spin hyperfine interactions by precision measurement of hyperfine structures of 127I2 near 532 nm

International Nuclear Information System (INIS)

Hong Fenglei; Zhang Yun; Ishikawa, Jun; Onae, Atsushi; Matsumoto, Hirokazu

2002-01-01

Hyperfine structures of the R(87)33-0, R(145)37-0, and P(132)36-0 transitions of molecular iodine near 532 nm are measured by observing the heterodyne beat-note signal of two I 2 -stabilized lasers, whose frequencies are bridged by an optical frequency comb generator. The measured hyperfine splittings are fit to a four-term Hamiltonian, which includes the electric quadrupole, spin-rotation, tensor spin-spin, and scalar spin-spin interactions, with an accuracy of ∼720 Hz. High-accurate hyperfine constants are obtained from this fit. Vibration dependences of the tensor spin-spin and scalar spin-spin hyperfine constants are determined for molecular iodine, for the first time to our knowledge. The observed hyperfine transitions are good optical frequency references in the 532-nm region

Phase transitions and molecular motions in [Ni(ND3)6](ClO4)2

International Nuclear Information System (INIS)

Migdal-Mikuli, Anna; Mikuli, Edward; Gorska, Natalia; Kowalska, Aneta; Ulanski, Jacek

2004-01-01

[Ni(ND 3 ) 6 ](ClO 4 ) 2 has three solid phases between 100 and 300 K. The phase transitions temperatures at heating (T C1 h =164.1 K and T C2 h =145.1 K) are shifted, as compared to the non-deuterated compound, towards the lower temperature of ca. 8 and 5 K, respectively. The ClO 4 - anions perform fast, picosecond, isotropic reorientation with the activation energy of 6.6 kJ mol -1 , which abruptly slow down at T C1 c phase transition, during sample cooling. The ND 3 ligands perform fast uniaxial reorientation around the Ni-N bond in all three detected phases, with the effective activation energy of 2.9 kJ mol -1 . The reorientational motion of ND 3 is only slightly distorted at the T C1 phase transition due to the dynamical orientational order-disorder process of anions. The low value of the activation energy for the ND 3 reorientation suggests that this reorientation undergoes the translation-rotation coupling, which makes the barrier to the rotation of the ammonia ligands not constant but fluctuating. The phase polymorphism and the dynamics of the molecular reorientations of the title compound are similar but not quite identical with these of the [Ni(NH 3 ) 6 ](ClO 4 ) 2

Reorientation of molecules in a Cl3P/Dirac h/NCCl2CF3 crystal according to NQR data

International Nuclear Information System (INIS)

Kyuntsel', I.A.; Mokeeva, V.A.; Soifer, G.B.

1988-01-01

The structural-dynamic inequivalence of the molecules in solid Cl 3 P/Dirac h/NCCl 2 CF 3 has been established, and their rotational mobility has been studied with the aid of the temperature dependence of the resonance frequency and of the spin-lattice relaxation time of the 35 Cl nuclei. The observed motion has been interpreted with consideration of the molecular structure as reorientation between unequal potential wells in the crystal lattice, and the corresponding activation parameters have been determined from the 35 Cl NQR data

Two-dimensional ferromagnet/semiconductor transition metal dichalcogenide contacts: p-type Schottky barrier and spin-injection control

KAUST Repository

Gan, Liyong; Cheng, Yingchun; Schwingenschlö gl, Udo; Zhang, Qingyun

2013-01-01

We study the ferromagnet/semiconductor contacts formed by transition metal dichalcogenide monolayers, focusing on semiconducting MoS2 and WS2 and ferromagnetic VS2. We investigate the degree of p-type doping and demonstrate tuning of the Schottky barrier height by vertical compressive pressure. An analytical model is presented for the barrier heights that accurately describes the numerical findings and is expected to be of general validity for all transition metal dichalcogenide metal/semiconductor contacts. Furthermore, magnetic proximity effects induce a 100% spin polarization at the Fermi level in the semiconductor where the spin splitting increases up to 0.70 eV for increasing pressure.

Two-dimensional ferromagnet/semiconductor transition metal dichalcogenide contacts: p-type Schottky barrier and spin-injection control

KAUST Repository

Gan, Liyong

2013-09-26

We study the ferromagnet/semiconductor contacts formed by transition metal dichalcogenide monolayers, focusing on semiconducting MoS2 and WS2 and ferromagnetic VS2. We investigate the degree of p-type doping and demonstrate tuning of the Schottky barrier height by vertical compressive pressure. An analytical model is presented for the barrier heights that accurately describes the numerical findings and is expected to be of general validity for all transition metal dichalcogenide metal/semiconductor contacts. Furthermore, magnetic proximity effects induce a 100% spin polarization at the Fermi level in the semiconductor where the spin splitting increases up to 0.70 eV for increasing pressure.

Spin glass transition in a thin-film NiO/permalloy bilayer

Science.gov (United States)

Ma, Tianyu; Urazhdin, Sergei

2018-02-01

We experimentally study magnetization aging in a thin-film NiO/permalloy bilayer. Aging characteristics are nearly independent of temperature below the exchange bias blocking temperature TB, but rapidly vary above it. The dependence on the magnetic history qualitatively changes across TB. The observed behaviors are consistent with the spin glass transition at TB, with significant implications for magnetism and magnetoelectronic phenomena in antiferromagnet/ferromagnet bilayers.

Characterization of domain reorientation in Pzt ceramics

International Nuclear Information System (INIS)

Lente, Manuel Henrique; Povoa, Jose Marques; Eiras, Jose Antonio

1997-01-01

The dynamic of domains in ferroelectric materials has been intensively studied due to its importance in applications like non volatile memories. Domain reorientation was characterized in lead zirconate titanate samples, pure and doped, through measurements of the transient current, after reversal a electric field. The reorientation behavior of the domains showed to be influenced by type of impurity (Nb or Fe) and by the electrical field intensity. Analysis of the experimental results reveals mainly the existence of two contributions: a dependent (t 0.1 s) of the field intensity. (author)

Nuclear reorientation in static and radio-frequency electro-magnetic fields

International Nuclear Information System (INIS)

Dubbers, D.

1976-01-01

Nuclear reorientation by external electromagnetic fields is treated using Fano's irreducible tensor formulation of the problem. Although the main purpose of this paper is the description of the effects of nuclear magnetic resonance (NMR) on an ensemble of oriented nuclei in the presence of a crystal electric field gradient (efg), the results are applicable to all types of nuclear or atomic orientation or angular correlation work. The theory is applied to a number of exemplary cases: magnetic field dependence of nuclear orientation in the presence of quadrupole interactions; sign determination in electric quadrupole coupling; line shapes of nuclear acoustic resonance (NAR) signals; quadrupole splitting and multiquantum transitions in NMR with oriented nuclei. (orig./WBU) [de

Multiple-Quantum Transitions and Charge-Induced Decoherence of Donor Nuclear Spins in Silicon

Science.gov (United States)

Franke, David P.; Pflüger, Moritz P. D.; Itoh, Kohei M.; Brandt, Martin S.

2017-06-01

We study single- and multiquantum transitions of the nuclear spins of an ensemble of ionized arsenic donors in silicon and find quadrupolar effects on the coherence times, which we link to fluctuating electrical field gradients present after the application of light and bias voltage pulses. To determine the coherence times of superpositions of all orders in the 4-dimensional Hilbert space, we use a phase-cycling technique and find that, when electrical effects were allowed to decay, these times scale as expected for a fieldlike decoherence mechanism such as the interaction with surrounding Si 29 nuclear spins.

Changing the cubic ferrimagnetic domain structure in temperature region of spin flip transition

International Nuclear Information System (INIS)

Djuraev, D.R.; Niyazov, L.N.; Saidov, K.S.; Sokolov, B.Yu.

2011-01-01

The transformation of cubic ferrimagnetic Tb 0.2 Y 2.8 Fe 5 O 12 domain structure has been studied by magneto optic method in the temperature region of spontaneous spin flip phase transition (SPT). It has been found that SPT occurs in a finite temperature interval where the coexistence of low- and high- temperature magnetic phase domains has observed. A character of domain structure evolution in temperature region of spin flip essentially depends on the presence of mechanical stresses in crystal. Interpretation of experimental results has been carried out within the framework of SPT theory for a cubic crystal. (authors)

Managerial strategies to reorient hospitals towards health promotion: lessons from organisational theory.

Science.gov (United States)

Röthlin, Florian

2013-01-01

Reorienting health services towards health promotion is one of the major health promotion strategies stipulated by the Ottawa Charter). Important contradictions, tensions and barriers to health promotion implementation associated with organisational structures have, thus far, been underexposed in the hospital health promotion discourse. This paper aims at identifying risks and the chances for hospital management to strategically and sustainably reorient their hospitals towards health promotion. The paper combines theories and findings from organisational science and management studies as well as from capacity development in the form of a narrative literature review. The aim is to focus on the conditions hospitals, as organisational systems with a highly professionalised workforce, provide for a strategically managed reorientation towards health promotion. Models and principles helping managers to navigate the difficulties and complexities of health promotion reorientation will be suggested. Hospital managers have to deal with genuine obstacles in the complexity and structural formation of hospital organisations. Against this background, continuous management support, a transformative leadership style, participative strategic management and expert governance can be considered important organisational capacities for the reorientation towards a new concept such as health promotion. This paper discusses managerial strategies, effective structural transformations and important organisational capacities that can contribute to a sustainable reorientation of hospitals towards health promotion. It supports hospital managers in exploring their chances of facilitating and effectively supporting a sustainable health promotion reorientation of their hospitals. The paper provides an innovative approach where the focus is on enhanced possibilities for hospital managers to strategically manage the reorientation towards health promotion.

Spin-chirality decoupling in Heisenberg spin glasses and related systems

OpenAIRE

Kawamura, Hikaru

2006-01-01

Recent studies on the spin and the chirality orderings of the three-dimensional Heisenberg spin glass and related systems are reviewed with particular emphasis on the possible spin-chirality decoupling phenomena. Chirality scenario of real spin-glass transition and its experimental consequence on the ordering of Heisenberg-like spin glasses are discussed.

Strain-induced phase transition and electron spin-polarization in graphene spirals.

Science.gov (United States)

Zhang, Xiaoming; Zhao, Mingwen

2014-07-16

Spin-polarized triangular graphene nanoflakes (t-GNFs) serve as ideal building blocks for the long-desired ferromagnetic graphene superlattices, but they are always assembled to planar structures which reduce its mechanical properties. Here, by joining t-GNFs in a spiral way, we propose one-dimensional graphene spirals (GSs) with superior mechanical properties and tunable electronic structures. We demonstrate theoretically the unique features of electron motion in the spiral lattice by means of first-principles calculations combined with a simple Hubbard model. Within a linear elastic deformation range, the GSs are nonmagnetic metals. When the axial tensile strain exceeds an ultimate strain, however, they convert to magnetic semiconductors with stable ferromagnetic ordering along the edges. Such strain-induced phase transition and tunable electron spin-polarization revealed in the GSs open a new avenue for spintronics devices.

Spin-dependent electronic transport properties of transition metal atoms doped α-armchair graphyne nanoribbons

Science.gov (United States)

Fotoohi, Somayeh; Haji-Nasiri, Saeed

2018-04-01

Spin-dependent electronic transport properties of single 3d transition metal (TM) atoms doped α-armchair graphyne nanoribbons (α-AGyNR) are investigated by non-equilibrium Green's function (NEGF) method combined with density functional theory (DFT). It is found that all of the impurity atoms considered in this study (Fe, Co, Ni) prefer to occupy the sp-hybridized C atom site in α-AGyNR, and the obtained structures remain planar. The results show that highly localized impurity states are appeared around the Fermi level which correspond to the 3d orbitals of TM atoms, as can be derived from the projected density of states (PDOS). Moreover, Fe, Co, and Ni doped α-AGyNRs exhibit magnetic properties due to the strong spin splitting property of the energy levels. Also for each case, the calculated current-voltage characteristic per super-cell shows that the spin degeneracy in the system is obviously broken and the current becomes strongly spin dependent. Furthermore, a high spin-filtering effect around 90% is found under the certain bias voltages in Ni doped α-AGyNR. Additionally, the structure with Ni impurity reveals transfer characteristic that is suitable for designing a spin current switch. Our findings provide a high possibility to design the next generation spin nanodevices with novel functionalities.

Influence of quantum phase transition on spin transport in the quantum antiferromagnet in the honeycomb lattice

Science.gov (United States)

Lima, L. S.

2017-06-01

We use the SU(3) Schwinger boson theory to study the spin transport properties of the two-dimensional anisotropic frustrated Heisenberg model in a honeycomb lattice at T = 0 with single ion anisotropy and third neighbor interactions. We have investigated the behavior of the spin conductivity for this model that presents exchange interactions J1 , J2 and J3 . We study the spin transport in the Bose-Einstein condensation regime where the bosons tz are condensed. Our results show an influence of the quantum phase transition point on the spin conductivity behavior. We also have made a diagrammatic expansion for the Green-function and did not obtain any significant change of the results.

Motional spin relaxation in photoexcited triplet states

International Nuclear Information System (INIS)

Harryvan, D.; Faassen, E. van

1997-01-01

Transient EPR experiments were performed on photoexcited spin triplet states of the luminescent dye EOSIN-Y in diluted (order of 1 nMol) frozen propane-1-ol solutions at various temperatures. Photoexcitation was achieved by irradiation with intense, short laser pulses. The details of the spin relaxation, in particular the dependence on time, magnetic field and microwave field strength are all reproduced by a model which computes the total magnetization in a population of photoexcited triplet states undergoing random reorientational motion. Using this model, we estimated the motional correlation times to be around a microsecond. This timescale is two orders of magnitude slower than the phase memory time of the triplets. (author)

Spin inelastic electron tunneling spectroscopy on local spin adsorbed on surface.

Science.gov (United States)

Fransson, J

2009-06-01

The recent experimental conductance measurements taken on magnetic impurities on metallic surfaces, using scanning tunneling microscopy technique and suggesting occurrence of inelastic scattering processes, are theoretically addressed. We argue that the observed conductance signatures are caused by transitions between the spin states that have opened due to, for example, exchange coupling between the local spins and the tunneling electrons, and are directly interpretable in terms of inelastic transitions energies. Feasible measurements using spin-polarized scanning tunneling microscopy that would enable new information about the excitation spectrum of the local spins are discussed.

Spin-Spin Cross Relaxation in Single-Molecule Magnets

Science.gov (United States)

Wernsdorfer, W.; Bhaduri, S.; Tiron, R.; Hendrickson, D. N.; Christou, G.

2002-10-01

The one-body tunnel picture of single-molecule magnets (SMMs) is not always sufficient to explain the measured tunnel transitions. An improvement to the picture is proposed by including also two-body tunnel transitions such as spin-spin cross relaxation (SSCR) which are mediated by dipolar and weak superexchange interactions between molecules. A Mn4 SMM is used as a model system. At certain external fields, SSCRs lead to additional quantum resonances which show up in hysteresis loop measurements as well-defined steps. A simple model is used to explain quantitatively all observed transitions.

Quasi-continuous transition from a Fermi liquid to a spin liquid in κ-(ET)2Cu2(CN)3.

Science.gov (United States)

Furukawa, Tetsuya; Kobashi, Kazuhiko; Kurosaki, Yosuke; Miyagawa, Kazuya; Kanoda, Kazushi

2018-01-22

The Mott metal-insulator transition-a manifestation of Coulomb interactions among electrons-is known as a discontinuous transition. Recent theoretical studies, however, suggest that the transition is continuous if the Mott insulator carries a spin liquid with a spinon Fermi surface. Here, we demonstrate the case of a quasi-continuous Mott transition from a Fermi liquid to a spin liquid in an organic triangular-lattice system κ-(ET) 2 Cu 2 (CN) 3 . Transport experiments performed under fine pressure tuning have found that as the Mott transition is approached, the Fermi liquid coherence temperature continuously falls to the scale of kelvins, with a divergent quasi-particle decay rate on the metal side, and the charge gap continuously closes on the insulator side. A Clausius-Clapeyron analysis provides thermodynamic evidence for the extremely weak first-order nature of the transition. These results provide additional support for the existence of a spinon Fermi surface, which becomes an electron Fermi surface when charges are delocalized.

Young children reorient by computing layout geometry, not by matching images of the environment.

Science.gov (United States)

Lee, Sang Ah; Spelke, Elizabeth S

2011-02-01

Disoriented animals from ants to humans reorient in accord with the shape of the surrounding surface layout: a behavioral pattern long taken as evidence for sensitivity to layout geometry. Recent computational models suggest, however, that the reorientation process may not depend on geometrical analyses but instead on the matching of brightness contours in 2D images of the environment. Here we test this suggestion by investigating young children's reorientation in enclosed environments. Children reoriented by extremely subtle geometric properties of the 3D layout: bumps and ridges that protruded only slightly off the floor, producing edges with low contrast. Moreover, children failed to reorient by prominent brightness contours in continuous layouts with no distinctive 3D structure. The findings provide evidence that geometric layout representations support children's reorientation.

Spin re-orientation in heavy fermion system α - YbAl1 - x FexB4

Science.gov (United States)

Wu, Shan; Broholm, C.; Kuga, K.; Suzuki, Shintaro; Nakatsuji, S.; Mourigal, M.; Stone, M.; Tian, Wei; Qiu, Y.; Rodriguez-Rivera, Jose

Non centro-symmetric α - YbAlB4 has a heavy Fermi liquid ground state and shares many characteristics with centro-symmetric β - YbAlB4 . Both isomorphs display intermediate valence, associated with a fluctuation scale of T0 = 200 K and a Kondo lattice scale of T* = 8 K. Unlike β - YbAlB4 , α - YbAlB4 is at the boundary of a transition from a Fermi liquid metallic state to an antiferromagnetic (AFM) insulating state, driven by Fe substitution of Al. Magnetization and specific heat measurements reveal two different antiferromagnetic phases with TN = 9 K and TN = 2 K for Fe concentration above and below x =0.07. We report single crystal neutron scattering experiments on Fe doped YbAlB4 with x =0.035 and x =0.125. While the ordering wave vector is identical, k -> = (1 , 0 , 0) , the spin orientation switches from c to a with increasing Fe concentration. This suggests different anisotropic hybridization between 4f and conduction electrons that we confirmed by determining the crystal field levels. Supported by DOE, BES through DE-FG02-08ER46544.

Monte Carlo simulations of phase transitions and lattice dynamics in an atom-phonon model for spin transition compounds

International Nuclear Information System (INIS)

Apetrei, Alin Marian; Enachescu, Cristian; Tanasa, Radu; Stoleriu, Laurentiu; Stancu, Alexandru

2010-01-01

We apply here the Monte Carlo Metropolis method to a known atom-phonon coupling model for 1D spin transition compounds (STC). These inorganic molecular systems can switch under thermal or optical excitation, between two states in thermodynamical competition, i.e. high spin (HS) and low spin (LS). In the model, the ST units (molecules) are linked by springs, whose elastic constants depend on the spin states of the neighboring atoms, and can only have three possible values. Several previous analytical papers considered a unique average value for the elastic constants (mean-field approximation) and obtained phase diagrams and thermal hysteresis loops. Recently, Monte Carlo simulation papers, taking into account all three values of the elastic constants, obtained thermal hysteresis loops, but no phase diagrams. Employing Monte Carlo simulation, in this work we obtain the phase diagram at T=0 K, which is fully consistent with earlier analytical work; however it is more complex. The main difference is the existence of two supplementary critical curves that mark a hysteresis zone in the phase diagram. This explains the pressure hysteresis curves at low temperature observed experimentally and predicts a 'chemical' hysteresis in STC at very low temperatures. The formation and the dynamics of the domains are also discussed.

Magnetic surface domain imaging of uncapped epitaxial FeRh(001) thin films across the temperature-induced metamagnetic transition

Energy Technology Data Exchange (ETDEWEB)

Zhou, Xianzhong; Matthes, Frank; Bürgler, Daniel E., E-mail: d.buergler@fz-juelich.de; Schneider, Claus M. [Peter Grünberg Institut, Electronic Properties (PGI-6) and Jülich-Aachen Research Alliance, Fundamentals of Future Information Technology (JARA-FIT), Forschungszentrum Jülich, D-52425 Jülich (Germany)

2016-01-15

The surface magnetic domain structure of uncapped epitaxial FeRh/MgO(001) thin films was imaged by in-situ scanning electron microscopy with polarization analysis (SEMPA) at various temperatures between 122 and 450 K. This temperature range covers the temperature-driven antiferromagnetic-to-ferromagnetic phase transition in the body of the films that was observed in-situ by means of the more depth-sensitive magneto-optical Kerr effect. The SEMPA images confirm that the interfacial ferromagnetism coexisting with the antiferromagnetic phase inside the film is an intrinsic property of the FeRh(001) surface. Furthermore, the SEMPA data display a reduction of the in-plane magnetization occuring well above the phase transition temperature which, thus, is not related to the volume expansion at the phase transition. This observation is interpreted as a spin reorientation of the surface magnetization for which we propose a possible mechanism based on temperature-dependent tetragonal distortion due to different thermal expansion coefficients of MgO and FeRh.

Spin reorientation and magnetoelastic properties of ferromagnetic T b1 -xN dxC o2 systems with a morphotropic phase boundary

Science.gov (United States)

Murtaza, Adil; Yang, Sen; Chang, Tieyan; Ghani, Awais; Khan, Muhammad Tahir; Zhang, Rui; Zhou, Chao; Song, Xiaoping; Suchomel, Matthew; Ren, Yang

2018-03-01

The spin reorientation (SR) and magnetoelastic properties of pseudobinary ferromagnetic T b1 -xN dxC o2 (0 ≤x ≤1.0 ) systems involving a morphotropic phase boundary (MPB) were studied by high-resolution synchrotron x-ray diffraction (XRD), magnetization, and magnetostriction measurements. The easy magnetization direction of the Laves phase lies along the 〈111 〉 axis with x 0.65 below Curie temperature (TC). The temperature-dependent magnetization curves showed SR; this can be explained by a two-sublattice model. Based on the synchrotron (XRD) and magnetization measurements, the SR phase diagram for a MPB composition of T b0.35N d0.65C o2 was obtained. Contrary to previously reported ferromagnetic systems involving MPB, the MPB composition of T b0.35N d0.65C o2 exhibits a low saturation magnetization (MS), indicating a compensation of the Tb and Nd magnetic moments at MPB. The anisotropic magnetostriction (λS) first decreased until x =0.8 and then continuously increased in the negative direction with further increase of Nd concentration. The decrease in magnetostriction can be attributed to the decrease of spontaneous magnetostriction λ111 and increase of λ100 with opposite sign to λ111. This paper indicates an anomalous type of MPB in the ferromagnetic T b1 -xN dxC o2 system and provides an active way to design novel functional materials with exotic properties.

Fundamental experiments on hydride reorientation in zircaloy

Science.gov (United States)

Colas, Kimberly B.

In the current study, an in-situ X-ray diffraction technique using synchrotron radiation was used to follow directly the kinetics of hydride dissolution and precipitation during thermomechanical cycles. This technique was combined with conventional microscopy (optical, SEM and TEM) to gain an overall understanding of the process of hydride reorientation. Thus this part of the study emphasized the time-dependent nature of the process, studying large volume of hydrides in the material. In addition, a micro-diffraction technique was also used to study the spatial distribution of hydrides near stress concentrations. This part of the study emphasized the spatial variation of hydride characteristics such as strain and morphology. Hydrided samples in the shape of tensile dog-bones were used in the time-dependent part of the study. Compact tension specimens were used during the spatial dependence part of the study. The hydride elastic strains from peak shift and size and strain broadening were studied as a function of time for precipitating hydrides. The hydrides precipitate in a very compressed state of stress, as measured by the shift in lattice spacing. As precipitation proceeds the average shift decreases, indicating average stress is reduced, likely due to plastic deformation and morphology changes. When nucleation ends the hydrides follow the zirconium matrix thermal contraction. When stress is applied below the threshold stress for reorientation, hydrides first nucleate in a very compressed state similar to that of unstressed hydrides. After reducing the average strain similarly to unstressed hydrides, the average hydride strain reaches a constant value during cool-down to room temperature. This could be due to a greater ease of deforming the matrix due to the applied far-field strain which would compensate for the strains due to thermal contraction. Finally when hydrides reorient, the average hydride strains become tensile during the first precipitation regime and

LANGUAGE REORIENTATION AND POLICY IMPLEMENTATION ...

African Journals Online (AJOL)

Chinwe Ugochukwu

building and leadership challenge; language reorientation; conclusion and ... Igbo land, for example, many students enrol to study foreign languages, but the reverse is the ... Following the lead of Franz Boas, such a view is no longer relevant. ... Consequently, on International Mother Language Day, all languages share.

Electric dipole spin resonance in a quantum spin dimer system driven by magnetoelectric coupling

Science.gov (United States)

Kimura, Shojiro; Matsumoto, Masashige; Akaki, Mitsuru; Hagiwara, Masayuki; Kindo, Koichi; Tanaka, Hidekazu

2018-04-01

In this Rapid Communication, we propose a mechanism for electric dipole active spin resonance caused by spin-dependent electric polarization in a quantum spin gapped system. This proposal was successfully confirmed by high-frequency electron spin resonance (ESR) measurements of the quantum spin dimer system KCuCl3. ESR measurements by an illuminating linearly polarized electromagnetic wave reveal that the optical transition between the singlet and triplet states in KCuCl3 is driven by an ac electric field. The selection rule of the observed transition agrees with the calculation by taking into account spin-dependent electric polarization. We suggest that spin-dependent electric polarization is effective in achieving fast control of quantum spins by an ac electric field.

Elementary excitations and the phase transition in the bimodal Ising spin glass model

International Nuclear Information System (INIS)

Jinuntuya, N; Poulter, J

2012-01-01

We show how the nature of the phase transition in the two-dimensional bimodal Ising spin glass model can be understood in terms of elementary excitations. Although the energy gap with the ground state is expected to be 4J in the ferromagnetic phase, a gap 2J is in fact found if the finite lattice is wound around a cylinder of odd circumference L. This 2J gap is really a finite size effect that should not occur in the thermodynamic limit of the ferromagnet. The spatial influence of the frustration must be limited and not wrap around the system if L is large enough. In essence, the absence of 2J excitations defines the ferromagnetic phase without recourse to calculating the magnetization or investigating the system response to domain wall defects. This study directly investigates the response to temperature. We also estimate the defect concentration where the phase transition to the spin glass state occurs. The value p c = 0.1045(11) is in reasonable agreement with the literature

Effect of silver nanoparticles on photo-induced reorientation of azo groups in polymer films

International Nuclear Information System (INIS)

Zhou Jingli; Yang Jianjun; Sun Youyi; Zhang Douguo; Shen Jing; Zhang Qijin; Wang Keyi

2007-01-01

A series of polymer films containing azo groups and silver nanoparticles were prepared. Photo-induced reorientation of the film was conducted under irradiation of polarized light with wavelength at 365 nm, 442 nm and 532 nm, respectively. The influence of the concentration of dopant silver on the reorientation of the azo groups was studied. An enhancement of about 50% for the reorientation rate and about 70% for the reorientation amplitude was achieved. From a comparison of the enhancement obtained by irradiating with three different light sources, it was realized that the mechanism for enhancement of reorientation of azo groups is due to plasmon resonance of silver nanoparticles doped in the polymer films

Moessbauer spectroscopy studies of spin reorientations in amorphous and crystalline (Co0.2Fe0.8)72.5Si12.5B15 glass coated micro-wires

International Nuclear Information System (INIS)

Nowik, I.; Felner, I.; Garcia-Miquel, H.

2007-01-01

Thermo-gravimetric, differential scanning calorimetry and comprehensive 57 Fe Moessbauer spectroscopy studies of amorphous and crystalline ferromagnetic glass coated (Co 0.2 Fe 0.8 ) 72.5 Si 12.5 B 15 micro-wires have been recorded. The Curie temperature of the amorphous phase is T C (amorp) ∼730 K. The analysis of the Moessbauer spectra reveals that below 623 K the easy axis of the magnetization is axial-along the wires, and that a tangential or/and radial orientation occurs at higher temperatures. At 770 K, in the first 4 hours the Moessbauer spectrum exhibits a pure paramagnetic doublet. Crystallization and decomposition to predominantly α-Fe(Si) and Fe 2 B occurs either by raising the temperature above 835 K or isothermally in time at lower temperatures. Annealing for a day at 770 K, leads to crystallization. In the crystalline material the magnetic moments have a complete random orientation. After cooling back to ambient temperature, both α-Fe(Si) and Fe 2 B in the glass coated wire show pure axial magnetic orientation like in the original amorphous state. The observed spin reorientations are associated with changes in the stress induced by the glass coating

Spin transitions in La{sub 0.7} Ba{sub 0.3}CoO{sub 3} thin films revealed by combining Raman spectroscopy and X-ray diffraction

Energy Technology Data Exchange (ETDEWEB)

Othmen, Zied; Oueslati, Meherzi [Unité Nanomatériaux et Photonique, Faculty of Sciences of Tunis, Tunis El-Manar University, 2092 Tunis (Tunisia); Copie, Olivier; Gemeiner, Pascale; Dkhil, Brahim [Laboratoire Structures, Propriétés et Modélisation des Solides, Centrale Supélec, CNRS-UMR 8580, Université Paris-Saclay (France); Daoudi, Kais [Unité Nanomatériaux et Photonique, Faculty of Sciences of Tunis, Tunis El-Manar University, 2092 Tunis (Tunisia); Department of Applied Physics and Astronomy, College of Sciences, University of Sharjah, P.O. Box 27272, Sharjah (United Arab Emirates); Boudard, Michel [Univ. Grenoble Alpes, LMGP, F-38000 Grenoble (France)

2016-07-07

In cobaltite, the spin states transitions of Co{sup 3+/4+} ions govern the magnetic and electronic conduction properties. These transitions are strain-sensitive and can be varied using external parameters, including temperature, hydrostatic pressure, or chemical stresses through ionic substitutions. In this work, using temperature dependent Raman spectroscopy and X-ray diffraction, the epitaxial strain effects on both structural and vibrational properties of La{sub 0.7} Ba{sub 0.3} CoO{sub 3} (LBCO) cobaltite thin films are investigated. All Raman active phonon modes as well as the structure are found to be strongly affected. Both Raman modes and lattice parameter evolutions show temperature changes correlated with magnetic and electronic transitions properties. Combining Raman spectroscopy and X-ray diffraction appears as a powerful approach to probe the spin transition in thin film cobaltite. Our results provide insight into strong spin-charge-phonon coupling in LBCO thin film. This coupling manifests as vibrational transition with temperature in the Raman spectra near the ferromagnetic spin ordered transition at 220 K.

Recent advances of spin crossover research

NARCIS (Netherlands)

Gutlich, P; van Koningsbruggen, PJ; Renz, F; Schonherr, T

2004-01-01

Thermal spin transition (spin crossover), one of the most fascinating dynamic electronic structure phenomena occurring in coordination compounds of third row transition metal ions, mostly of iron(II), iron(III) and cobalt(II) with critical ligand field strengths competing with the spin pairing

Tectonic patterns on a reoriented planet - Mars

International Nuclear Information System (INIS)

Melosh, H.J.

1980-01-01

Both geological and free-air-gravity data suggest that the positive mass anomaly associated with the Tharsis volcanoes may have reoriented Mars' lithosphere by as much as 25 deg. Since Mars is oblate, rotation of the lithosphere over the equatorial bulge by 25 deg produces membrane stresses of several kilobars, large enough to initiate faulting. Plots of the magnitude and direction of stresses in a reoriented planet show that near Tharsis the dominant fault type should be north-south-trending normal faults. This normal fault province is centered at 30 deg N latitude and extends about 45 deg east and west in longitude. Similar faults should occur at the antipodes, north of Hellas Planitia

Determination of the physical parameters distribution in spin transition compounds using experimental FORC diagram

International Nuclear Information System (INIS)

Tanasa, Radu; Linares, Jorge; Enachescu, Cristian; Varret, Francois; Stancu, Alexandru

2006-01-01

Spin transitions materials are characterized with an innovative experimental method, i.e. first-order reversal curve (FORC) diagram. The interpretation of the results is performed in the framework of two different Ising-like models: a mean-field approach and the exact solution done by the Monte Carlo entropic sampling (MCES) method

Field-induced strain memory with non-180 .deg. domain-reorientation control

International Nuclear Information System (INIS)

Kadota, Yoichi; Hosaka, Hiroshi; Morita, Takeshi

2010-01-01

Using non-180 .deg. domain-reorientation control, we propose the strain memory effect in ferroelectric ceramics. Electric fields with asymmetric amplitudes were applied to soft-type lead zirconate titanate (PZT) ceramics, and the strain hysteresis and the polarization loop were measured. The butterfly curve became asymmetric under an electric field with a particular asymmetric amplitude. The asymmetric butterfly curve had two stable strain states at zero electric field. Thus, the strain memory effect was realized as the difference between the two stable strain states. An XRD analysis was carried out to verify the contribution of the non-180 .deg. domain reorientation to the strain memory effect. The non-180 .deg. domain reorientation was determined as the intensity ratio of the (002) to the (200) peak. The strain memory determined from macroscopic strain measurements had a linear relationship to the non-180 .deg. domain volume fraction. This result indicated the origin of the strain memory to be the non-180 .deg. domain reorientation.

Planar reorientation maneuvers of space multibody systems using internal controls

Science.gov (United States)

Reyhanoglu, Mahmut; Mcclamroch, N. H.

1992-01-01

In this paper a reorientation maneuvering strategy for an interconnection of planar rigid bodies in space is developed. It is assumed that there are no exogeneous torques, and torques generated by joint motors are used as means of control so that the total angular momentum of the multibody system is a constant, assumed to be zero in this paper. The maneuver strategy uses the nonintegrability of the expression for the angular momentum. We demonstrate that large-angle maneuvers can be designed to achieve an arbitrary reorientation of the multibody system with respect to an inertial frame. The theoretical background for carrying out the required maneuvers is briefly summarized. Specifications and computer simulations of a specific reorientation maneuver, and the corresponding control strategies, are described.

A magnetic relaxation study on anisotropic reorientation in aqueous polyelectrolyte solutions

International Nuclear Information System (INIS)

Mulder, C.W.R.

1984-01-01

The present thesis proposes a study on anisotropic reorientation of aqueous polyelectrolyte solutions. In particular, it is directed to the question to what extent information may be obtained on anisotropic reorientation by nuclear magnetic relaxation experiments. The polymethacrylic acid/water system has been chosen as probe system. (Auth.)

The Nuclear Spin Nanomagnet

OpenAIRE

Korenev, V. L.

2007-01-01

Linearly polarized light tuned slightly below the optical transition of the negatively charged exciton (trion) in a single quantum dot causes the spontaneous nuclear spin polarization (self-polarization) at a level close to 100%. The effective magnetic field of spin-polarized nuclei brings the optical transition energy into resonance with photon energy. The resonantly enhanced Overhauser effect sustains the stability of the nuclear self-polarization even in the absence of spin polarization of...

Transitions in eigenvalue and wavefunction structure in (1+2) -body random matrix ensembles with spin.

Science.gov (United States)

Vyas, Manan; Kota, V K B; Chavda, N D

2010-03-01

Finite interacting Fermi systems with a mean-field and a chaos generating two-body interaction are modeled by one plus two-body embedded Gaussian orthogonal ensemble of random matrices with spin degree of freedom [called EGOE(1+2)-s]. Numerical calculations are used to demonstrate that, as lambda , the strength of the interaction (measured in the units of the average spacing of the single-particle levels defining the mean-field), increases, generically there is Poisson to GOE transition in level fluctuations, Breit-Wigner to Gaussian transition in strength functions (also called local density of states) and also a duality region where information entropy will be the same in both the mean-field and interaction defined basis. Spin dependence of the transition points lambda_{c} , lambdaF, and lambdad , respectively, is described using the propagator for the spectral variances and the formula for the propagator is derived. We further establish that the duality region corresponds to a region of thermalization. For this purpose we compared the single-particle entropy defined by the occupancies of the single-particle orbitals with thermodynamic entropy and information entropy for various lambda values and they are very close to each other at lambda=lambdad.

Spin-exchange interaction between transition metals and metalloids in soft-ferromagnetic metallic glasses

Science.gov (United States)

Das, Santanu; Choudhary, Kamal; Chernatynskiy, Aleksandr; Choi Yim, Haein; Bandyopadhyay, Asis K.; Mukherjee, Sundeep

2016-06-01

High-performance magnetic materials have immense industrial and scientific importance in wide-ranging electronic, electromechanical, and medical device technologies. Metallic glasses with a fully amorphous structure are particularly suited for advanced soft-magnetic applications. However, fundamental scientific understanding is lacking for the spin-exchange interaction between metal and metalloid atoms, which typically constitute a metallic glass. Using an integrated experimental and molecular dynamics approach, we demonstrate the mechanism of electron interaction between transition metals and metalloids. Spin-exchange interactions were investigated for a Fe-Co metallic glass system of composition [(Co1-x Fe x )0.75B0.2Si0.05]96Cr4. The saturation magnetization increased with higher Fe concentration, but the trend significantly deviated from simple rule of mixtures. Ab initio molecular dynamics simulation was used to identify the ferromagnetic/anti-ferromagnetic interaction between the transition metals and metalloids. The overlapping band-structure and density of states represent ‘Stoner type’ magnetization for the amorphous alloys in contrast to ‘Heisenberg type’ in crystalline iron. The enhancement of magnetization by increasing iron was attributed to the interaction between Fe 3d and B 2p bands, which was further validated by valence-band study.

In Situ AFM Imaging of Microstructural Changes Associated with The Spin Transition in [Fe(Htrz)₂(Trz)](Bf₄) Nanoparticles.

Science.gov (United States)

Manrique-Juárez, María D; Suleimanov, Iurii; Hernández, Edna M; Salmon, Lionel; Molnár, Gábor; Bousseksou, Azzedine

2016-06-30

Topographic images of [Fe(Htrz)₂(trz)](BF₄) nanoparticles were acquired across the first-order spin transition using variable-temperature atomic force microscopy (AFM) in amplitude modulation mode. These studies revealed a complex morphology of the particles consisting of aggregates of small nanocrystals, which expand, separate and re-aggregate due to the mechanical stress during the spin-state switching events. Both reversible (prompt or slow recovery) and irreversible effects (fatigue) on the particle morphology were evidenced and correlated with the spin crossover properties.

Spatial reorientation by geometry in bumblebees.

Directory of Open Access Journals (Sweden)

Valeria Anna Sovrano

Full Text Available Human and non-human animals are capable of using basic geometric information to reorient in an environment. Geometric information includes metric properties associated with spatial surfaces (e.g., short vs. long wall and left-right directionality or 'sense' (e.g. a long wall to the left of a short wall. However, it remains unclear whether geometric information is encoded by explicitly computing the layout of surface geometry or by matching images of the environment. View-based spatial encoding is generally thought to hold for insect navigation and, very recently, evidence for navigation by geometry has been reported in ants but only in a condition which does not allow the animals to use features located far from the goal. In this study we tested the spatial reorientation abilities of bumblebees (Bombus terrestris. After spatial disorientation, by passive rotation both clockwise and anticlockwise, bumblebees had to find one of the four exit holes located in the corners of a rectangular enclosure. Bumblebees systematically confused geometrically equivalent exit corners (i.e. corners with the same geometric arrangement of metric properties and sense, for example a short wall to the left of a long wall. However, when one wall of the enclosure was a different colour, bumblebees appeared to combine this featural information (either near or far from the goal with geometric information to find the correct exit corner. Our results show that bumblebees are able to use both geometric and featural information to reorient themselves, even when features are located far from the goal.

Control of electron spin decoherence in nuclear spin baths

Science.gov (United States)

Liu, Ren-Bao

2011-03-01

Nuclear spin baths are a main mechanism of decoherence of spin qubits in solid-state systems, such as quantum dots and nitrogen-vacancy (NV) centers of diamond. The decoherence results from entanglement between the electron and nuclear spins, established by quantum evolution of the bath conditioned on the electron spin state. When the electron spin is flipped, the conditional bath evolution is manipulated. Such manipulation of bath through control of the electron spin not only leads to preservation of the center spin coherence but also demonstrates quantum nature of the bath. In an NV center system, the electron spin effectively interacts with hundreds of 13 C nuclear spins. Under repeated flip control (dynamical decoupling), the electron spin coherence can be preserved for a long time (> 1 ms) . Thereforesomecharacteristicoscillations , duetocouplingtoabonded 13 C nuclear spin pair (a dimer), are imprinted on the electron spin coherence profile, which are very sensitive to the position and orientation of the dimer. With such finger-print oscillations, a dimer can be uniquely identified. Thus, we propose magnetometry with single-nucleus sensitivity and atomic resolution, using NV center spin coherence to identify single molecules. Through the center spin coherence, we could also explore the many-body physics in an interacting spin bath. The information of elementary excitations and many-body correlations can be extracted from the center spin coherence under many-pulse dynamical decoupling control. Another application of the preserved spin coherence is identifying quantumness of a spin bath through the back-action of the electron spin to the bath. We show that the multiple transition of an NV center in a nuclear spin bath can have longer coherence time than the single transition does, when the classical noises due to inhomogeneous broadening is removed by spin echo. This counter-intuitive result unambiguously demonstrates the quantumness of the nuclear spin bath

Large magnetocaloric effect of NdGa compound due to successive magnetic transitions

Science.gov (United States)

Zheng, X. Q.; Xu, J. W.; Shao, S. H.; Zhang, H.; Zhang, J. Y.; Wang, S. G.; Xu, Z. Y.; Wang, L. C.; Chen, J.; Shen, B. G.

2018-05-01

The magnetic behavior and MCE property of NdGa compound were studied in detail. According to the temperature dependence of magnetization (M-T) curve at 0.01 T, two sharp changes were observed at 20 K (TSR) and 42 K (TC), respectively, corresponding to spin reorientation and FM-PM transition. Isothermal magnetization curves up to 5 T at different temperatures were measured and magnetic entropy change (ΔSM) was calculated based on M-H data. Temperature dependences of -ΔSM for a field change of 0-2 T and 0-5 T show that there are two peaks on the curves corresponding to TSR and TC, respectively. The value of the two peaks is 6.4 J/kg K and 15.5 J/kg K for the field change of 0-5 T. Since the two peaks are close, the value of -ΔSM in the temperature range between TSR and TC keeps a large value. The excellent MCE performance of NdGa compound benefits from the existence of two successive magnetic transitions.

Evidence for two spin-glass transitions with magnetoelastic and magnetoelectric couplings in the multiferroic (B i1 -xB ax) (F e1 -xT ix ) O3 system

Science.gov (United States)

Kumar, Arun; Kaushik, S. D.; Siruguri, V.; Pandey, Dhananjai

2018-03-01

For disordered Heisenberg systems with small single ion anisotropy (D ), two spin-glass (SG) transitions below the long-range ordered (LRO) phase transition temperature (Tc) have been predicted theoretically for compositions close to the percolation threshold. Experimental verification of these predictions is still controversial for conventional spin glasses. We show that multiferroic spin-glass systems can provide a unique platform for verifying these theoretical predictions via a study of change in magnetoelastic and magnetoelectric couplings, obtained from an analysis of diffraction data, at the spin-glass transition temperatures (TSG). Results of macroscopic (dc M (H , T ), M(t ), ac susceptibility [χ (ω, T )], and specific heat (Cp)) and microscopic (x-ray and neutron scattering) measurements are presented on disordered BiFe O3 , a canonical Heisenberg system with small single ion anisotropy, which reveal appearance of two spin-glass phases, SG1 and SG2, in coexistence with the LRO phase below the Almeida-Thouless (A-T) and Gabey-Toulouse (G-T) lines. It is shown that the temperature dependence of the integrated intensity of the antiferromagnetic (AFM) peak shows dips with respect to the Brillouin function behavior around the SG1 and SG2 transition temperatures. The temperature dependence of the unit cell volume departs from the Debye-Grüneisen behavior below the SG1 transition and the magnitude of departure increases significantly with decreasing temperature up to the electromagnon driven transition temperature below which a small change of slope occurs followed by another similar change of slope at the SG2 transition temperature. The ferroelectric polarization also changes significantly at the two spin-glass transition temperatures. These results, obtained using microscopic techniques, clearly demonstrate that the SG1 and SG2 transitions occur on the same magnetic sublattice and are intrinsic to the system. We also construct a phase diagram showing all

Integer Quantum Magnon Hall Plateau-Plateau Transition in a Spin Ice Model

OpenAIRE

Xu, Baolong; Ohtsuki, Tomi; Shindou, Ryuichi

2016-01-01

Low-energy magnon bands in a two-dimensional spin ice model become integer quantum magnon Hall bands. By calculating the localization length and the two-terminal conductance of magnon transport, we show that the magnon bands with disorders undergo a quantum phase transition from an integer quantum magnon Hall regime to a conventional magnon localized regime. Finite size scaling analysis as well as a critical conductance distribution shows that the quantum critical point belongs to the same un...

Evidence for a temperature-induced spin-state transition of Co3+ in La2-xSrxCoO4

Science.gov (United States)

Hollmann, N.; Haverkort, M. W.; Benomar, M.; Cwik, M.; Braden, M.; Lorenz, T.

2011-05-01

We study the magnetic susceptibility of mixed-valent La2-xSrxCoO4 single crystals in the doping range of 0.5⩽x⩽0.8 for temperatures up to 1000 K. The magnetism below room temperature is described by paramagnetic Co2+ in the high-spin state and by Co3+ in the nonmagnetic low-spin state. At high temperatures, an increase in susceptibility is seen, which we attribute to a temperature-induced spin-state transition of Co3+. The susceptibility is analyzed by comparison to full-multiplet calculations for the thermal population of the high- and intermediate-spin states of Co3+.

Evidence of spin transition and charge order in cobalt substituted La sub 0 sub . sub 7 Ca sub 0 sub . sub 3 MnO sub 3

CERN Document Server

Srivastava, C M; Gundurao, T K; Nigam, A K; Bahadur, D

2003-01-01

The transport and magnetic studies of a series of compounds having the general formula La sub 0 sub . sub 7 Ca sub 0 sub . sub 3 Mn sub 1 sub - sub x Co sub x O sub 3 (0.1 = 0.25 there is a clear spin transition at low temperature from the high to the low spin state of trivalent cobalt and this leads to change in ferromagnetic (FM) and antiferromagnetic (AFM) phases. For x >= 0.25 there are two transitions for each value of x: the upper one gives the FM and AFM spin arrangement depending upon whether the DE or the SE dominates; the lower one is obtained due to the transition from the high to the low spin state of the trivalent cobalt ion.

Visually induced reorientation illusions

Science.gov (United States)

Howard, I. P.; Hu, G.; Oman, C. M. (Principal Investigator)

2001-01-01

It is known that rotation of a furnished room around the roll axis of erect subjects produces an illusion of 360 degrees self-rotation in many subjects. Exposure of erect subjects to stationary tilted visual frames or rooms produces only up to 20 degrees of illusory tilt. But, in studies using static tilted rooms, subjects remained erect and the body axis was not aligned with the room. We have revealed a new class of disorientation illusions that occur in many subjects when placed in a 90 degrees or 180 degrees tilted room containing polarised objects (familiar objects with tops and bottoms). For example, supine subjects looking up at a wall of the room feel upright in an upright room and their arms feel weightless when held out from the body. We call this the levitation illusion. We measured the incidence of 90 degrees or 180 degrees reorientation illusions in erect, supine, recumbent, and inverted subjects in a room tilted 90 degrees or 180 degrees. We report that reorientation illusions depend on the displacement of the visual scene rather than of the body. However, illusions are most likely to occur when the visual and body axes are congruent. When the axes are congruent, illusions are least likely to occur when subjects are prone rather than supine, recumbent, or inverted.

Transit time corrected arterial spin labeling technique aids to overcome delayed transit time effect

International Nuclear Information System (INIS)

Yun, Tae Jin; Sohn, Chul-Ho; Yoo, Roh-Eul; Kang, Kyung Mi; Choi, Seung Hong; Kim, Ji-hoon; Park, Sun-Won; Hwang, Moonjung; Lebel, R.M.

2018-01-01

This study aimed to evaluate the usefulness of transit time corrected cerebral blood flow (CBF) maps based on multi-phase arterial spin labeling MR perfusion imaging (ASL-MRP). The Institutional Review Board of our hospital approved this retrospective study. Written informed consent was waived. Conventional and multi-phase ASL-MRPs and dynamic susceptibility contrast MR perfusion imaging (DSC-MRP) were acquired for 108 consecutive patients. Vascular territory-based volumes of interest were applied to CBF and time to peak (TTP) maps obtained from DSC-MRP and CBF maps obtained from conventional and multi-phase ASL-MRPs. The concordances between normalized CBF (nCBF) from DSC-MRP and nCBF from conventional and transition time corrected CBF maps from multi-phase ASL-MRP were evaluated using Bland-Altman analysis. In addition, the dependence of difference between nCBF (ΔnCBF) values obtained from DSC-MRP and conventional ASL-MRP (or multi-phase ASL-MRP) on TTP obtained from DSC-MRP was also analyzed using regression analysis. The values of nCBFs from conventional and multi-phase ASL-MRPs had lower values than nCBF based on DSC-MRP (mean differences, 0.08 and 0.07, respectively). The values of ΔnCBF were dependent on TTP values from conventional ASL-MRP technique (F = 5.5679, P = 0.0384). No dependency of ΔnCBF on TTP values from multi-phase ASL-MRP technique was revealed (F = 0.1433, P > 0.05). The use of transit time corrected CBF maps based on multi-phase ASL-MRP technique can overcome the effect of delayed transit time on perfusion maps based on conventional ASL-MRP. (orig.)

Transit time corrected arterial spin labeling technique aids to overcome delayed transit time effect

Energy Technology Data Exchange (ETDEWEB)

Yun, Tae Jin; Sohn, Chul-Ho; Yoo, Roh-Eul; Kang, Kyung Mi; Choi, Seung Hong; Kim, Ji-hoon [Seoul National University Medical Research Center, Institute of Radiation Medicine, Seoul (Korea, Republic of); Seoul National University Hospital, Department of Radiology, Seoul (Korea, Republic of); Park, Sun-Won [Seoul National University Medical Research Center, Institute of Radiation Medicine, Seoul (Korea, Republic of); Seoul National University Boramae Medical Center, Department of Radiology, Seoul (Korea, Republic of); Hwang, Moonjung [GE Healthcare Korea, Seoul (Korea, Republic of); Lebel, R.M. [GE Healthcare Canada, Calgary (Canada)

2018-03-15

This study aimed to evaluate the usefulness of transit time corrected cerebral blood flow (CBF) maps based on multi-phase arterial spin labeling MR perfusion imaging (ASL-MRP). The Institutional Review Board of our hospital approved this retrospective study. Written informed consent was waived. Conventional and multi-phase ASL-MRPs and dynamic susceptibility contrast MR perfusion imaging (DSC-MRP) were acquired for 108 consecutive patients. Vascular territory-based volumes of interest were applied to CBF and time to peak (TTP) maps obtained from DSC-MRP and CBF maps obtained from conventional and multi-phase ASL-MRPs. The concordances between normalized CBF (nCBF) from DSC-MRP and nCBF from conventional and transition time corrected CBF maps from multi-phase ASL-MRP were evaluated using Bland-Altman analysis. In addition, the dependence of difference between nCBF (ΔnCBF) values obtained from DSC-MRP and conventional ASL-MRP (or multi-phase ASL-MRP) on TTP obtained from DSC-MRP was also analyzed using regression analysis. The values of nCBFs from conventional and multi-phase ASL-MRPs had lower values than nCBF based on DSC-MRP (mean differences, 0.08 and 0.07, respectively). The values of ΔnCBF were dependent on TTP values from conventional ASL-MRP technique (F = 5.5679, P = 0.0384). No dependency of ΔnCBF on TTP values from multi-phase ASL-MRP technique was revealed (F = 0.1433, P > 0.05). The use of transit time corrected CBF maps based on multi-phase ASL-MRP technique can overcome the effect of delayed transit time on perfusion maps based on conventional ASL-MRP. (orig.)

Nuclear magnetic resonance in solids: evolution of spin temperature under multipulse irradiation and high symmetry molecular motions

International Nuclear Information System (INIS)

Quiroga, Luis

1982-01-01

In a first part, autocorrelation functions are calculated taking into account the symmetry of molecular motions by group theoretical techniques. This very general calculation method is then used to evaluate the NMR spin-lattice relaxation times T 1 and T 1 p as a function of the relative orientations of the magnetic field, the crystal and the rotation axis, in particular for cyclic, dihedral and cubic groups. Models of molecular reorientations such as jumps between a finite number of allowed orientations, rotational diffusion and superimposed reorientations are all investigated with the same formalism. In part two, the effect of the coherent excitation of spins, by multipulse sequences of the WHH-4 type, on the evolution of the heat capacity and spin temperature of the dipolar reservoir is analysed. It is shown both theoretically and experimentally that adiabatic (reversible) reduction of the dipolar Hamiltonian and its spin temperature is obtained when the amplitude of pulses (rotation angle) is slowly raised. The sudden switching on and off of the HW-8 sequence is then shown to lead to the same reversible reduction in a shorter time. It is also shown that, by this way, sensibility and selectivity of double resonance measurements of weak gyromagnetic ratio nuclei are strongly increased. This is experimentally illustrated in some cases. (author) [fr

Field induced phase transition in layered honeycomb spin system α-RuCl3 studied by thermal conductivity

Science.gov (United States)

Leahy, Ian; Bornstein, Alex; Choi, Kwang-Yong; Lee, Minhyea

α -RuCl3, a quasi -two-dimensional honeycomb lattice is known to be a candidate material to realize the Heisenberg-Kitaev spin model of a highly anisotropic bond-dependent exchange interaction. We investigate in-plane thermal conductivity (κ) as a function of temperature (T) and in-plane applied field (H). At H = 0 , the onset of a strong increase in κ marks the spontaneous long range ordering temperature, Tc = 6 . 5 K , corresponding to ``zigzag'' antiferromagnetic ordering. A broad peak appearing below Tc in κ was found to be suppressed significantly as H increases up to ~ 7 T , implying the system undergoes a field-induced transition from ordered to a new spin-disordered state analogous to the transverse-field Ising model. Further increasing H above 7 . 1 T , the large field seems to begin polarizing spins thus increasing the phonon mean free path, resulting in a significant rise in κ. This tendency is clearly shown in the field dependence of κ below Tc, which has a pronounced minimum at Hmin = 7 . 1 T . We will discuss our scaling analysis to characterize this field-induced phase transition and compare to the transverse-field Ising spin system. Work at the University of Colorado was supported by the US DOE Basic Energy Sciences under Award No. DE-SC0006888.

Mixed spin-3/2 and spin-5/2 Ising system on the Bethe lattice

International Nuclear Information System (INIS)

Albayrak, Erhan; Yigit, Ali

2006-01-01

In order to study the critical behaviors of the half-integer mixed spin-3/2 and spin-5/2 Blume-Capel Ising ferrimagnetic system, we have used the exact recursion relations on the Bethe lattice. The system was studied for the coordination numbers with q=3, 4, 5 and 6, and the obtained phase diagrams are illustrated on the (kT c /|J|,D A /|J|) plane for constant values of D B /|J|, the reduced crystal field of the sublattice with spin-5/2, and on the (kT c /|J|,D B /|J|) plane for constant values of D A /|J|, the reduced crystal field of the sublattice with spin-3/2, for q=3 only, since the cases corresponding to q=4, 5 and 6 reproduce results similar to the case for q=3. In addition we have also presented the phase diagram with equal strengths of the crystal fields for q=3, 4, 5 and 6. Besides the second- and first-order phase transitions, the system also exhibits compensation temperatures for appropriate values of the crystal fields. In this mixed spin system while the second-order phase transition lines never cut the reduced crystal field axes as in the single spin type spin-3/2 and spin-5/2 Ising models separately, the first-order phase transition lines never connect to the second-order phase transition lines and they end at the critical points, therefore the system does not give any tricritical points. In addition to this, this mixed-spin model exhibits one or two compensation temperatures depending on the values of the crystal fields, as a result the compensation temperature lines show reentrant behavior

Molecular reorientation of dye doped nematic liquid crystals in the laser illumination

International Nuclear Information System (INIS)

San, S. E.; Koeysal, O.; Ecevit, F. N.

2002-01-01

In this study it is investigated how dye doped nematic liquid crystals reorient under the illumination of laser beam whose wavelength is appropriate to absorbance characteristics of the doping dye. Nematic liquid crystal E7 is used with anthraquinone dye 1% wt/wt in the preparation of the sample and this material is filled in homegenously aligned measurement cell having 15 μm thickness. Mechanism of molecular reorientation includes the absorbance effects of the energy of laser by doping dye and this reorientation causes the refractive index of the material to be changed. There are potential application possibilities of such molecular reorientation based effects in nonlinear optics such as real time holography whose basis is grating diffraction that is observed and investigated in the frame of fundamentals of molecule light interaction mechanisms. Experimental analyses allowed finding characteristic values of diffraction signals depending on physical parameters of set up for a dye doped liquid crystal system and this system provided a 20 % diffraction efficiency under the optimum circumstances

Structural anomalies, spin transitions and charge disproportionation in LnCoO.sub.3./sub..

Czech Academy of Sciences Publication Activity Database

Knížek, Karel; Jirák, Zdeněk; Hejtmánek, Jiří; Henry, P.; André, G.

2008-01-01

Roč. 103, č. 7 (2008), 07B703/1-07B703/3 ISSN 0021-8979 R&D Projects: GA ČR GA202/06/0051 Institutional research plan: CEZ:AV0Z10100521 Keywords : LnCoO 3 * neutron diffraction * thermal expansion * spin-state transition Subject RIV: BM - Solid Matter Physics ; Magnetism Impact factor: 2.201, year: 2008

Spin nematics next to spin singlets

Science.gov (United States)

Yokoyama, Yuto; Hotta, Chisa

2018-05-01

We provide a route to generate nematic order in a spin-1/2 system. Unlike the well-known magnon-binding mechanism, our spin nematics requires neither the frustration effect nor spin polarization in a high field or in the vicinity of a ferromagnet, but instead appears next to the spin singlet phase. We start from a state consisting of a quantum spin-1/2 singlet dimer placed on each site of a triangular lattice, and show that interdimer ring exchange interactions efficiently dope the SU(2) triplets that itinerate and interact, easily driving a stable singlet state to either Bose-Einstein condensates or a triplet crystal, some hosting a spin nematic order. A variety of roles the ring exchange serves includes the generation of a bilinear-biquadratic interaction between nearby triplets, which is responsible for the emergent nematic order separated from the singlet phase by a first-order transition.

Electron spin torque in atoms

International Nuclear Information System (INIS)

Hara, Takaaki; Senami, Masato; Tachibana, Akitomo

2012-01-01

The spin torque and zeta force, which govern spin dynamics, are studied by using monoatoms in their steady states. We find nonzero local spin torque in transition metal atoms, which is in balance with the counter torque, the zeta force. We show that d-orbital electrons have a crucial effect on these torques. Nonzero local chirality density in transition metal atoms is also found, though the electron mass has the effect to wash out nonzero chirality density. Distribution patterns of the chirality density are the same for Sc–Ni atoms, though the electron density distributions are different. -- Highlights: ► Nonzero local spin torque is found in the steady states of transition metal atoms. ► The spin steady state is realized by the existence of a counter torque, zeta force. ► D-orbital electrons have a crucial effect on the spin torque and zeta force. ► Nonzero local chiral density is found in spite of the washout by the electron mass. ► Chiral density distribution have the same pattern for Sc–Ni atoms.

Electronic Structure from Iron L-edge Spectroscopy : An Example of Spin Transition Evidenced by Soft X-ray Absorption Spectroscopy

NARCIS (Netherlands)

Cartier dit Moulin, Ch.; Flank, A.M.; Rudolf, P.; Chen, C.T.

1993-01-01

Soft X-ray Absorption Spectroscopy at the transition metal L2,3 edges provides information about the 3d unoccupied states by dipole allowed transitions. We have recorded iron L2,3 edges in order to follow the reversible thermal spin interconversion (S=2 S=0) of the Fe(II)(o-phenantroline)2(NCS)2.

Understanding the spin-driven polarizations in Bi MO3 (M = 3 d transition metals) multiferroics

Science.gov (United States)

Kc, Santosh; Lee, Jun Hee; Cooper, Valentino R.

Bismuth ferrite (BiFeO3) , a promising multiferroic, stabilizes in a perovskite type rhombohedral crystal structure (space group R3c) at room temperature. Recently, it has been reported that in its ground state it possess a huge spin-driven polarization. To probe the underlying mechanism of this large spin-phonon response, we examine these couplings within other Bi based 3 d transition metal oxides Bi MO3 (M = Ti, V, Cr, Mn, Fe, Co, Ni) using density functional theory. Our results demonstrate that this large spin-driven polarization is a consequence of symmetry breaking due to competition between ferroelectric distortions and anti-ferrodistortive octahedral rotations. Furthermore, we find a strong dependence of these enhanced spin-driven polarizations on the crystal structure; with the rhombohedral phase having the largest spin-induced atomic distortions along [111]. These results give us significant insights into the magneto-electric coupling in these materials which is essential to the magnetic and electric field control of electric polarization and magnetization in multiferroic based devices. Research is supported by the US Department of Energy, Office of Science, Basic Energy Sciences, Materials Science and Engineering Division and the Office of Science Early Career Research Program (V.R.C) and used computational resources at NERSC.

Scaling of quantum Fisher information close to the quantum phase transition in the XY spin chain

Energy Technology Data Exchange (ETDEWEB)

Ye, En-Jia, E-mail: yeenjia@jiangnan.edu.cn [Jiangsu Provincial Research Center of Light Industrial Optoelectronic Engineering and Technology, School of Science, Jiangnan University, Wuxi 214122 (China); Hu, Zheng-Da [Jiangsu Provincial Research Center of Light Industrial Optoelectronic Engineering and Technology, School of Science, Jiangnan University, Wuxi 214122 (China); Wu, Wei [Zhejiang Institute of Modern Physics and Physics Department, Zhejiang University, Hangzhou 310027 (China)

2016-12-01

The quantum phase transition of an XY spin chain is investigated by employing the quantum Fisher information encoded in the ground state. It is shown that the quantum Fisher information is an effective tool for characterizing the quantum criticality. The quantum Fisher information, its first and second derivatives versus the transverse field display the phenomena of sudden transition, sudden jump and divergence, respectively. Besides, the analysis of finite size scaling for the second derivative of quantum Fisher information is performed.

Study on gamma-ray transitions induced in nuclear spin isomers by X-rays

International Nuclear Information System (INIS)

Yang Tianli; Hao Fanhua; Liu Xiaoya; Gong Jian

2005-10-01

The development of induced X-ray has been summarized for high spin isomer. the radiation model, transition mechanism and experiment plan have been introduced. The experiments about isomers 180m Ta and 178m2 Hf have been narrated in detail respectively, and the analysis between those results have been obtained. The reasonable theoretical frame and good experimental data have offered the powerful technique base for pumping γ-ray laser with low energy. (authors)

Pressure effect on hysteresis in spin-crossover solid materials

Energy Technology Data Exchange (ETDEWEB)

Gudyma, Iurii, E-mail: yugudyma@gmail.com [Department of General Physics, Chernivtsi National University, Chernivtsi 58012 (Ukraine); Ivashko, Victor [Department of General Physics, Chernivtsi National University, Chernivtsi 58012 (Ukraine); Dimian, Mihai [Department of Electrical and Computer Engineering, Howard University, Washington DC 20059 (United States); Faculty of Electrical Engineering and Computer Science & Integrated Center for Research, Development and Innovation in Advanced Materials, Nanotechnologies, and Distributed Systems for fabrication and control, Stefan cel Mare University, Suceava 720229 (Romania)

2016-04-01

A generalized microscopic Ising-like model is proposed to describe behavior of compressible spin-crossover solids with two states: low-spin and high-spin. The model was solved in mean-field approximation and shows hysteretic behavior at low energy difference between the states. We study the thermal transition between states under external hydrostatic pressure taking into account the changes in the volume of spin-crossover molecules in different states. Depending on the applied pressure, a spin-crossover system can have three types of behavior of molecular fraction in the high-spin state: hysteretic, second-order phase transition and no-phase transition. For the hysteretic regime, it is shown that the transition temperature under pressure is increased while the width of the hysteresis reduced.

Spin relaxation near the metal-insulator transition: dominance of the Dresselhaus spin-orbit coupling.

Science.gov (United States)

Intronati, Guido A; Tamborenea, Pablo I; Weinmann, Dietmar; Jalabert, Rodolfo A

2012-01-06

We identify the Dresselhaus spin-orbit coupling as the source of the dominant spin-relaxation mechanism in the impurity band of a wide class of n-doped zinc blende semiconductors. The Dresselhaus hopping terms are derived and incorporated into a tight-binding model of impurity sites, and they are shown to unexpectedly dominate the spin relaxation, leading to spin-relaxation times in good agreement with experimental values. This conclusion is drawn from two complementary approaches: an analytical diffusive-evolution calculation and a numerical finite-size scaling study of the spin-relaxation time.

A new high-pressure phase of Fe2SiO4 and the relationship between spin and structural transitions

Science.gov (United States)

Yamanaka, T.; Kyono, A.; Nakamoto, Y.; Kharlamova, S. A.; Struzhkin, V. V.; Gramsch, S.; Mao, H.; Hemley, R. J.

2013-12-01

Structure transformation of Fe2SiO4 Angle-dispersive powder x-ray diffraction was carried out at beam line 16-BMD APS. Structure of a new high-pressure phase of I-Fe2SiO4 spinel was determined by Rietveld profile fitting of x-ray diffraction data up to 64GPa at ambient temperature. A structural transition from the cubic spinel to the new structure was observed at 34GPa. Diffraction patterns taken at 44.6GPa and 54.6GPa indicate a two-phase mixture of spinel and new high-pressure phase. Reversible transition from I-Fe2SiO4 to spinel was confirmed. Laser heating experiment at 1500K proved the decomposition of Fe2SiO4 spinel to two oxides of FeO and SiO2. Spin transition X-ray emission measurements of Fe2SiO4 were carried out up to 65GPa at ambient temperature at beam line 16-IDD APS. The spin transition exerts an influence to Fe2SiO4 spinel structure and triggers two distinct curves of the lattice constant in the spinel phase. Although the compression curve of the spinel is discontinuous at approximately 20 GPa, Fe Kβ emission measurements show that the transition from a high spin (HS) to an intermediate spin (IS) state begins at 17GPa in the spinel phase. The IS electronic state is gradually enhanced with pressure, which results in an isostructural phase transition. HS-to-LS transition of iron bearing spinels starts from 15.6GPa in Fe3O4 and 19.6GPa in Fe2TiO4. The transition is more capable due to Fe2+ in the octahedral site. The extremely shortened octahedral bonds result in a distortion of 6-fold cation site. New structure of Fe2SiO4 Monte Carlo method was applied to find candidates for the high-pressure phase using the diffraction intensities with fixed lattice constants determined by DICVOL. Rietveld profile fitting was then performed using the initial model. The new structure is a body centered orthorhombic phase (I-Fe2SiO4) with space group Imma and Z=4, with two crystallographically distinct FeO6 octahedra. Silicon exists in six-fold coordination in I-Fe2Si

On the possibility of contact-induced spin polarization in interfaces of armchair nanotubes with transition metal substrates

Energy Technology Data Exchange (ETDEWEB)

Kuzubov, Alexander A. [Siberian Federal University, 79 Svobodny Prospect, 660041 Krasnoyarsk (Russian Federation); Kirensky Institute of Physics, 50 Akademgorodok, 660036 Krasnoyarsk (Russian Federation); Kovaleva, Evgenia A., E-mail: kovaleva.evgeniya1991@mail.ru [Siberian Federal University, 79 Svobodny Prospect, 660041 Krasnoyarsk (Russian Federation); Kirensky Institute of Physics, 50 Akademgorodok, 660036 Krasnoyarsk (Russian Federation); Tomilin, Felix N.; Mikhaleva, Natalya S.; Kuklin, Artem V. [Siberian Federal University, 79 Svobodny Prospect, 660041 Krasnoyarsk (Russian Federation); Kirensky Institute of Physics, 50 Akademgorodok, 660036 Krasnoyarsk (Russian Federation)

2015-12-15

The interaction between armchair carbon and boron nitride nanotubes (NT) with ferromagnetic transition metal (TM) surfaces, namely, Ni(111) and Co(0001), was studied by means of density functional theory. Different configurations of composite compartments mutual arrangement were considered. Partial densities of states and spin density spatial distribution of optimized structures were investigated. Influence of ferromagnetic substrate on nanotubes’ electronic properties was discussed. The values of spin polarization magnitude at the Fermi level are also presented and confirm the patterns of spin density spatial distribution. - Highlights: • Interaction of armchair nanotubes with ferromagnetic metal surfaces was investigated. • Different configurations of nanotube's location were considered. • For all nanotubes the energy difference between configurations is negligible. • Nanotubes were found to be more or less spin-polarized regarding to the configuration. • BN nanotubes demonstrate vanishing of the band gap and contact-induced conductivity.

Spin Transition in the Lower Mantle: Deep Learning and Pattern Recognition of Superplumes from the Mid-mantle and Mid-mantle Slab Stagnation

Science.gov (United States)

Yuen, D. A.; Shahnas, M. H.; De Hoop, M. V.; Pysklywec, R.

2016-12-01

The broad, slow seismic anomalies under Africa and Pacific cannot be explained without ambiguity. There is no well-established theory to explain the fast structures prevalent globally in seismic tomographic images that are commonly accepted to be the remnants of fossil slabs at different depths in the mantle. The spin transition from high spin to low spin in iron in ferropericlase and perovskite, two major constituents of the lower mantle can significantly impact their physical properties. We employ high resolution 2D-axisymmetric and 3D-spherical control volume models to reconcile the influence of the spin transition-induced anomalies in density, thermal expansivity, and bulk modulus in ferropericlase and perovskite on mantle dynamics. The model results reveal that the spin transition effects increase the mixing in the lower regions of mantle. Depending on the changes of bulk modulus associated with the spin transition, these effects may also cause both stagnation of slabs and rising plumes at mid-mantle depths ( 1600 km). The stagnation may be followed by downward or upward penetration of cold or hot mantle material, respectively, through an avalanche process. The size of these mid-mantle plumes reaches 1500 km across with a radial velocity reaching 20 cm/yr near the seismic transition zone and plume heads exceeding 2500 km across. We will employ a deep-learning algorithm to formulate this challenge as a classification problem where modelling/computation aids in the learning stage for detecting the particular patterns.The parameters based on which the convection models are developed are poorly constrained. There are uncertainties in initial conditions, heterogeneities and boundary conditions in the simulations, which are nonlinear. Thus it is difficult to reconstruct the past configuration over long time scales. In order to extract information and better understand the parameters in mantle convection, we employ deep learning algorithm to search for different

The effect of stress state on zirconium hydride reorientation

Science.gov (United States)

Cinbiz, Mahmut Nedim

correlating the finite element stress-state results with the spatial distribution of hydride microstructures observed within the optical micrographs for each sample. Experiments showed that the hydride reorientation was enhanced as the stress biaxiality increased. The threshold stress decreased from 150 MPa to 80 MPa when stress biaxiality ratio increased from uniaxial tension to near-equibiaxial tension. This behavior was also predicted by classical nucleation theory based on the Gibbs free energy of transformation being assisted by the far-field stress. An analysis of in situ X-ray diffraction data obtained during a thermo-mechanical cycle typical of vacuum drying showed a complex lattice-spacing behavior of the hydride phase during the dissolution and precipitation. The in-plane hydrides showed bilinear lattice expansion during heating with the intrinsic thermal expansion rate of the hydrides being observed only at elevated temperatures as they dissolve. For radial hydrides that precipitate during cooling under stress, the spacing of the close-packed {111} planes oriented normal to the maximum applied stress was permanently higher than the corresponding {111} plane spacing in the other directions. This behavior is believed to be a result of a complex stress state within the precipitating plate-like hydrides that induces a strain component within the hydrides normal to its "plate" face (i.e., the applied stress direction) that exceeds the lattice spacing strains in the other directions. During heat-up, the lattice spacing of these same "plate" planes actually contract due to the reversion of the stress state within the plate-like hydrides as they dissolve. The presence of radial hydrides and their connectivity with in-plane hydrides was shown to increase the ductile-to-brittle transition temperature during tensile testing. This behavior can be understood in terms of the role of radial hydrides in promoting the initiation of a long crack that subsequently propagates under

Thermocapillary reorientation of Janus drops

Science.gov (United States)

Rosales, Rodolfo; Saenz, Pedro

2017-11-01

Janus drops, named after the Ancient Roman two-faced god, are liquid drops formed from two immiscible fluids. Experimental observations indicate that a Janus drop may re-orientate in response to an applied external thermal gradient due to the Marangoni effect. Depending on the angle between the interior interface and the direction of the temperature gradient, disparities in the physical properties of the constituent liquids may lead to asymmetries in the thermocapillary flow. As a result, the drop will move along a curved path until a torque-free configuration is achieved, point after which it will continue on a straight trajectory. Here, we present the results of a theoretical investigation of this realignment phenomenon in the Stokes regime and in the limit of non-deformable interfaces. A 3D semi-analytical method in terms of polar spherical harmonics is developed to characterize and rationalize the hydrodynamic response (forces and torques), flow (velocity and temperature distribution) and trajectory of a Janus drop moving during the temperature-driven reorientation process. Furthermore, we discuss how this phenomenon may be exploited to develop dynamically reconfigurable micro-lenses. This work was partially supported by the US National Science Foundation through Grants DMS-1614043 and DMS-1719637.

High temperature spin-glass-like transition in La0.67Sr0.33MnO3 nanofibers near the Curie point.

Science.gov (United States)

Lu, Ruie; Yang, Sen; Li, Yitong; Chen, Kaiyun; Jiang, Yun; Fu, Bi; Zhang, Yin; Zhou, Chao; Xu, Minwei; Zhou, Xuan

2017-06-28

The glassy transition of superparamagnetic (SPM) (r glass-like (SGL) behavior near the Curie point (T C ), i.e., T 0 = 330 K, in La 0.67 Sr 0.33 MnO 3 (LSMO) nanofibers (NFs) composed of nanoparticles beyond the SPM size (r ≫ r 0 ), resulting in a significant increase of the glass transition temperature. This SGL transition near the T C of bulk LSMO can be explained to be the scenario of locally ordered clusters embedded in a disordered host, in which the assembly of nanoparticles has a magnetic core-shell model driven by surface spin glass. The presence of a surface spin glass of nanoparticles was proved by the Almeida-Thouless line δT f ∝ H 2/3 , exchange bias, and reduced saturation magnetization of the NF system. Composite dynamics were found - that is, both the SPM and the super-spin-glass (SSG) behavior are found in such an NF system. The bifurcation of the zero-field-cooled (ZFC) and field-cooled (FC) magnetization vs. temperature curves at the ZFC peak, and the flatness of FC magnetization involve SSG, while the frequency-dependent ac susceptibility anomaly follows the Vogel-Fulcher law that implies weak dipole interactions of the SPM model. This finding can help us to find a way to search for high temperature spin glass materials.

Relaxation theory of spin-3/2 Ising system near phase transition temperatures

International Nuclear Information System (INIS)

Canko, Osman; Keskin, Mustafa

2010-01-01

Dynamics of a spin-3/2 Ising system Hamiltonian with bilinear and biquadratic nearest-neighbour exchange interactions is studied by a simple method in which the statistical equilibrium theory is combined with the Onsager's theory of irreversible thermodynamics. First, the equilibrium behaviour of the model in the molecular-field approximation is given briefly in order to obtain the phase transition temperatures, i.e. the first- and second-order and the tricritical points. Then, the Onsager theory is applied to the model and the kinetic or rate equations are obtained. By solving these equations three relaxation times are calculated and their behaviours are examined for temperatures near the phase transition points. Moreover, the z dynamic critical exponent is calculated and compared with the z values obtained for different systems experimentally and theoretically, and they are found to be in good agrement. (general)

Mixed spin Ising model with four-spin interaction and random crystal field

International Nuclear Information System (INIS)

Benayad, N.; Ghliyem, M.

2012-01-01

The effects of fluctuations of the crystal field on the phase diagram of the mixed spin-1/2 and spin-1 Ising model with four-spin interactions are investigated within the finite cluster approximation based on a single-site cluster theory. The state equations are derived for the two-dimensional square lattice. It has been found that the system exhibits a variety of interesting features resulting from the fluctuation of the crystal field interactions. In particular, for low mean value D of the crystal field, the critical temperature is not very sensitive to fluctuations and all transitions are of second order for any value of the four-spin interactions. But for relatively high D, the transition temperature depends on the fluctuation of the crystal field, and the system undergoes tricritical behaviour for any strength of the four-spin interactions. We have also found that the model may exhibit reentrance for appropriate values of the system parameters.

Surface role in reorientation of internal layers of molybdenum single crystal during rolling

International Nuclear Information System (INIS)

Antsiforov, P.N.; Gorordetskij, S.D.; Markashova, A.I.; Martynenko, S.I.

1991-01-01

Structure, orientations and chemical composition of surface and internal layers of molybdenum rolled monocrystals are studied using electron microscopy, X-ray and Auger-analyses. Model of reorientation allowing to determine relation of deformation mechanism localized in surface layer with reorientation of internal layers, is described to explain the results

Heisenberg spin glass experiments and the chiral ordering scenario

International Nuclear Information System (INIS)

Campbell, Ian A.; Petit, Dorothee C.M.C.

2010-01-01

An overview is given of experimental data on Heisenberg spin glass materials so as to make detailed comparisons with numerical results on model Heisenberg spin glasses, with particular reference to the chiral driven ordering transition scenario due to Kawamura and collaborators. On weak anisotropy systems, experiments show critical exponents which are very similar to those estimated numerically for the model Heisenberg chiral ordering transition but which are quite different from those at Ising spin glass transitions. Again on weak anisotropy Heisenberg spin glasses, experimental torque data show well defined in-field transverse ordering transitions up to strong applied fields, in contrast to Ising spin glasses where fields destroy ordering. When samples with stronger anisotropies are studied, critical and in-field behavior tend progressively towards the Ising limit. It can be concluded that the essential physics of laboratory Heisenberg spin glasses mirrors that of model Heisenberg spin glasses, where chiral ordering has been demonstrated numerically. (author)

Large spin relaxation anisotropy and valley-Zeeman spin-orbit coupling in WSe2/graphene/h -BN heterostructures

Science.gov (United States)

Zihlmann, Simon; Cummings, Aron W.; Garcia, Jose H.; Kedves, Máté; Watanabe, Kenji; Taniguchi, Takashi; Schönenberger, Christian; Makk, Péter

2018-02-01

Large spin-orbital proximity effects have been predicted in graphene interfaced with a transition-metal dichalcogenide layer. Whereas clear evidence for an enhanced spin-orbit coupling has been found at large carrier densities, the type of spin-orbit coupling and its relaxation mechanism remained unknown. We show an increased spin-orbit coupling close to the charge neutrality point in graphene, where topological states are expected to appear. Single-layer graphene encapsulated between the transition-metal dichalcogenide WSe2 and h -BN is found to exhibit exceptional quality with mobilities as high as 1 ×105 cm2 V-1 s-1. At the same time clear weak antilocalization indicates strong spin-orbit coupling, and a large spin relaxation anisotropy due to the presence of a dominating symmetric spin-orbit coupling is found. Doping-dependent measurements show that the spin relaxation of the in-plane spins is largely dominated by a valley-Zeeman spin-orbit coupling and that the intrinsic spin-orbit coupling plays a minor role in spin relaxation. The strong spin-valley coupling opens new possibilities in exploring spin and valley degree of freedom in graphene with the realization of new concepts in spin manipulation.

Wetting and layering transitions of a spin-1/2 Ising model in a random transverse field

International Nuclear Information System (INIS)

Bahmad, L.; Benyoussef, A.; El-Kenz, A.; Ez-Zahraouy, H.

2000-09-01

The effect of a random transverse field (RTF) on the wetting and layering transitions of a spin-1/2 Ising model, in the presence of bulk and surface fields, is studied within an effective field theory by using the differential operator technique. Indeed, the dependencies of the wetting temperature and wetting transverse field on the probability of the presence of a transverse field are established. For specific values of the surface field we show the existence of a critical probability p, above which wetting and layering transitions disappear. (author)

Theory of relaxation phenomena in a spin-3/2 Ising system near the second-order phase transition temperature

International Nuclear Information System (INIS)

Keskin, Mustafa; Canko, Osman

2005-01-01

The relaxation behavior of the spin-3/2 Ising model Hamiltonian with bilinear and biquadratic interactions near the second-order phase transition temperature or critical temperature is studied by means of the Onsager's theory of irreversible thermodynamics or the Onsager reciprocity theorem (ORT). First, we give the equilibrium case briefly within the molecular-field approximation in order to study the relaxation behavior by using the ORT. Then, the ORT is applied to the model and the kinetic equations are obtained. By solving these equations, three relaxation times are calculated and examined for temperatures near the second-order phase transition temperature. It is found that one of the relaxation times goes to infinity near the critical temperature on either side, the second relaxation time makes a cusp at the critical temperature and third one behaves very differently in which it terminates at the critical temperature while approaching it, then showing a 'flatness' property and then decreases. We also study the influences of the Onsager rate coefficients on the relaxation times. The behavior of these relaxation times is discussed and compared with the spin-1/2 and spin-1 Ising systems

Anisotropic magnetic structures of the Mn R MnSbO6 high-pressure doubly ordered perovskites (R =La , Pr, and Nd)

Science.gov (United States)

Solana-Madruga, Elena; Arévalo-López, Ángel M.; Dos santos-García, Antonio J.; Ritter, Clemens; Cascales, Concepción; Sáez-Puche, Regino; Attfield, J. Paul

2018-04-01

A new type of doubly ordered perovskite (also reported as double double perovskite, DDPv) structure combining columnar and rock-salt orders of the cations at the A and B sites, respectively, was recently found at high pressure for Mn R MnSb O6 (R =La -Sm ). Here we report further magnetic structures of these compounds. M n2 + spins align into antiparallel ferromagnetic sublattices along the x axis for MnLaMnSb O6 , while the magnetic anisotropy of P r3 + magnetic moments induces their preferential order along the z direction for MnPrMnSb O6 . The magnetic structure of MnNdMnSb O6 was reported to show a spin-reorientation transition of M n2 + spins from the z axis towards the x axis driven by the ordering of N d3 + magnetic moments. The crystal-field parameters for P r3 + and N d3 + at the 4 e C2 site of their DDPv structure have been semiempirically estimated and used to derive their energy levels and associated wave functions. The results demonstrate that the spin-reorientation transition in MnNdMnSb O6 arises as a consequence of the crystal-field-induced magnetic anisotropy of N d3 + .

Observation of the anisotropic spin-glass transition and transverse spin ordering in pseudo-brookite through muon spin relaxation

NARCIS (Netherlands)

Boekema, C.; Brabers, V.A.M.; Lichti, R.L.; Denison, A.B.; Cooke, D.W.; Heffner, R.H.; Hutson, R.L.; Schillaci, M.E.; MacLaughlin, D.E.; Dodds, S.A.

1986-01-01

Zero-field longitudinal muon-spin-relaxation (µSR) experiments have been performed on single crystals of pseudo-brookite (Fe2-xTil+x O 5; x=0.25), an anisotropic spin-glass system. The spinglass temperature (Tg) is determined to be 44.0±0.5K. Above Tg, a distinct exponential muon-spin-relaxation

Quantum Monte Carlo studies of a metallic spin-density wave transition

Energy Technology Data Exchange (ETDEWEB)

Gerlach, Max Henner

2017-01-20

Plenty experimental evidence indicates that quantum critical phenomena give rise to much of the rich physics observed in strongly correlated itinerant electron systems such as the high temperature superconductors. A quantum critical point of particular interest is found at the zero-temperature onset of spin-density wave order in two-dimensional metals. The appropriate low-energy theory poses an exceptionally hard problem to analytic theory, therefore the unbiased and controlled numerical approach pursued in this thesis provides important contributions on the road to comprehensive understanding. After discussing the phenomenology of quantum criticality, a sign-problem-free determinantal quantum Monte Carlo approach is introduced and an extensive toolbox of numerical methods is described in a self-contained way. By the means of large-scale computer simulations we have solved a lattice realization of the universal effective theory of interest. The finite-temperature phase diagram, showing both a quasi-long-range spin-density wave ordered phase and a d-wave superconducting dome, is discussed in its entirety. Close to the quantum phase transition we find evidence for unusual scaling of the order parameter correlations and for non-Fermi liquid behavior at isolated hot spots on the Fermi surface.

Tuning the Magnetic Anisotropy at a Molecule-Metal Interface

DEFF Research Database (Denmark)

Bairagi, K.; Bellec, A.; Repain, V.

2015-01-01

We demonstrate that a C60 overlayer enhances the perpendicular magnetic anisotropy of a Co thin film, inducing an inverse spin reorientation transition from in plane to out of plane. The driving force is the C60/Co interfacial magnetic anisotropy that we have measured quantitatively in situ...

Dynamic Phase Transitions In The Spin-2 Ising System Under An Oscillating Magnetic Field Within The Effective-Field Theory

International Nuclear Information System (INIS)

Ertas, Mehmet; Keskin, Mustafa; Deviren, Bayram

2010-01-01

The dynamic phase transitions are studied in the spin-2 Ising model under a time-dependent oscillating magnetic field by using the effective-field theory with correlations. The effective-field dynamic equation is derived by employing the Glauber transition rates and the phases in the system are obtained by solving this dynamic equation. The nature (first- or second-order) of the dynamic phase transition is characterized by investigating the thermal behavior of the dynamic order parameter and the dynamic phase transition temperatures are obtained. The dynamic phase diagrams are presented in (T/zJ, h/zJ) plane.

Analytical description of spin-Rabi oscillation controlled electronic transitions rates between weakly coupled pairs of paramagnetic states with S=(1)/(2)

Science.gov (United States)

Glenn, R.; Baker, W. J.; Boehme, C.; Raikh, M. E.

2013-04-01

We report on the theoretical and experimental study of spin-dependent electronic transition rates which are controlled by a radiation-induced spin-Rabi oscillation of weakly spin-exchange and spin-dipolar coupled paramagnetic states (S=(1)/(2)). The oscillation components [the Fourier content, F(s)] of the net transition rates within spin-pair ensembles are derived for randomly distributed spin resonances, with an account of a possible correlation between the two distributions corresponding to individual pair partners. Our study shows that when electrically detected Rabi spectroscopy is conducted under an increasing driving field B1, the Rabi spectrum, F(s), evolves from a single peak at s=ΩR, where ΩR=γB1 is the Rabi frequency (γ is the gyromagnetic ratio), to three peaks at s=ΩR, s=2ΩR, and low s≪ΩR. The crossover between the two regimes takes place when ΩR exceeds the expectation value δ0 of the difference in the Zeeman energies within the pairs, which corresponds to the broadening of the magnetic resonance by disorder caused by a hyperfine field or distributions of Landé g factors. We capture this crossover by analytically calculating the shapes of all three peaks at an arbitrary relation between ΩR and δ0. When the peaks are well developed their widths are Δs˜δ02/ΩR. We find a good quantitative agreement between the theory and experiment.

Spin glass transition in the rhombohedral LiNi1/3Mn1/3Co1/3O2

International Nuclear Information System (INIS)

Bie, Xiaofei; Yang, Xu; Han, Bing; Chen, Nan; Liu, Lina; Wei, Yingjin; Wang, Chunzhong; Chen, Hong; Du, Fei; Chen, Gang

2013-01-01

Highlights: •The Rietveld analysis of XRD data reveals a single phase with rhombohedral structure. •Dc susceptibility data suggest a spin glass behavior at low T in the 333 compound. •The ac susceptibility measurements have been observed in the typical SG system. •Three models have been employed to study the behavior of the spin glass state. •Both geometrical frustration and disorder play important role in the formation of SG. -- Abstract: Layered LiNi 1/3 Mn 1/3 Co 1/3 O 2 has been synthesized by co-precipitation method, and the magnetic properties were comprehensively studied by dc and ac susceptibilities. The dc magnetization curves show the irreversibility and spin freezing behavior at 109 K and 9 K. The evolution of real and imaginary part of ac susceptibility under different frequencies indicates a spin glass transition at low temperature. Three models (the Néel–Arrhenius law, the Vogel–Fulcher law, and the power law) have been employed to study the relaxation behavior of the spin glass state. Both frustration and disorder play important role in the formation of spin glass

Effect of Noise on the Decoherence of a Central Electron Spin Coupled to an Antiferromagnetic Spin Bath

Directory of Open Access Journals (Sweden)

G. C. Fouokeng

2014-01-01

Full Text Available We analyze the influence of a two-state autocorrelated noise on the decoherence and on the tunneling Landau-Zener (LZ transitions during a two-level crossing of a central electron spin (CES coupled to a one dimensional anisotropic-antiferomagnetic spin, driven by a time-dependent global external magnetic field. The energy splitting of the coupled spin system is found through an approach that computes the noise-averaged frequency. At low magnetic field intensity, the decoherence (or entangled state of a coupled spin system is dominated by the noise intensity. The effects of the magnetic field pulse and the spin gap antiferromagnetic material used suggest to us that they may be used as tools for the direct observation of the tunneling splitting through the LZ transitions in the sudden limit. We found that the dynamical frequencies display basin-like behavior decay with time, with the birth of entanglement, while the LZ transition probability shows Gaussian shape.

Graphene on transition-metal dichalcogenides: a platform for proximity spin-orbit physics and optospintronics

OpenAIRE

Gmitra, Martin; Fabian, Jaroslav

2015-01-01

Hybrids of graphene and two dimensional transition metal dichalcogenides (TMDC) have the potential to bring graphene spintronics to the next level. As we show here by performing first-principles calculations of graphene on monolayer MoS$_2$, there are several advantages of such hybrids over pristine graphene. First, Dirac electrons in graphene exhibit a giant global proximity spin-orbit coupling, without compromising the semimetallic character of the whole system at zero field. Remarkably, th...

Hysteretic behavior of spin-crossover noise driven system

Energy Technology Data Exchange (ETDEWEB)

Gudyma, Iurii [Department of General Physics, Chernivtsi National University, Chernivtsi 58012 (Ukraine); Maksymov, Artur, E-mail: maxyartur@gmail.com [Department of General Physics, Chernivtsi National University, Chernivtsi 58012 (Ukraine); Advanced Materials Research Institute, University of New Orleans, LA 70148 (United States); Dimian, Mihai [Department of Electrical and Computer Engineering, Howard University, Washington DC, 20059 (United States); Faculty of Electrical Engineering and Computer Science, Stefan cel Mare University, Suceava 720229 (Romania)

2016-04-01

The influence of white Gaussian noise on hysteretic behavior of spin-crossover system is analyzed in the framework of stochastic Langevin dynamics. Various stochastic simulations are performed and several important properties of spin-transition in spin-crossover system driven by noise are reproduced. The numerical results are tested against the stationary probability function and the associated dynamic potential obtained from Fokker–Planck equation corresponding to spin-crossover Langevin dynamics. The dependence of light-induced optical hysteresis width and non-hysteretic transition curve slope on the noise intensity is illustrated. The role of low-spin and high-spin phase stabilities in the hysteretic behavior of noise-driven spin-crossover system is discussed.

Mixed-Spin Diamond Chain Cu2FePO4F4(H2O)4 with a Noncollinear Spin Order and Possible Successive Phase Transitions.

Science.gov (United States)

Lu, Hongcheng; Hayashi, Naoaki; Matsumoto, Yuki; Takatsu, Hiroshi; Kageyama, Hiroshi

2017-08-07

A diamond spin chain system, one of the one-dimensional frustrated lattices, is known to exhibit novel properties, but experimental studies have been exclusively confined to materials with a single spin component. Here, we report on the synthesis, structure, and magnetic properties of a new diamond chain compound Cu 2 FePO 4 F 4 (H 2 O) 4 1 composed of mixed-spins of Cu 2+ (S = 1/2 × 2) and Fe 3+ (S = 5/2). Compound 1 crystallizes in the space group C2/c of the monoclinic crystal system with a = 7.7546(4) Å, b = 12.1290(6) Å, c = 9.9209(6) Å, β = 105.29(1)°, and Z = 4. DC magnetization, Mössbauer spectroscopy, and heat capacity measurements revealed an antiferromagnetic order at 11.3 K with a small ferromagnetic component. It is suggested that ferrimagnetic diamond chains are arranged in an antiferromagnetic fashion (i.e., [...Fe(↑)-2Cu(↓↓)-Fe(↑)...] and [...Fe(↓)-2Cu(↑↑)-Fe(↓)...]) within the ab plane to cancel net magnetization, and the spin orientation of the diamond chains changes alternately along the c axis due to the magnetic anisotropy, leading to a noncollinear spin order. Furthermore, another anomaly is observed in the heat capacity at around 3 K, suggesting a successive magnetic transition or crossover due to competing magnetic interactions.

Quantum Fidelity and Thermal Phase Transitions in a Two-Dimensional Spin System

International Nuclear Information System (INIS)

Wang Bo; Kou Su-Peng; Huang Hai-Lin; Sun Zhao-Yu

2012-01-01

We investigate the ability of quantum fidelity in detecting the classical phase transitions (CPTs) in a two-dimensional Heisenberg—Ising mixed spin model, which has a very rich phase diagram and is exactly soluble. For a two-site subsystem of the model, the reduced fidelity (including the operator fidelity and the fidelity susceptibility) at finite temperatures is calculated, and it is found that an extreme value presents at the critical temperature, thus shows a signal for the CPTs. In some parameter region, the signal becomes blurred. We propose to use the 'normalized fidelity susceptibility' to solve this problem

Pressure response of vacancy ordered maghemite (γ-Fe2O3) and high pressure transformed hematite (α-Fe2O3)

International Nuclear Information System (INIS)

Hearne, Giovanni; Pischedda, Vittoria

2012-01-01

Combined XRD and Mössbauer effect spectroscopy studies to high pressures of ∼30 GPa of vacancy ordered maghemite are presented. The vacancy ordered superstructure is robust and remains intact up to the pressure-induced onset transition to hematite at 13–16 GPa. The pressure transformed hematite is shown to be crystallographically textured, unlike the randomised low pressure maghemite phase. This arises out of a pressure or stress instigated topotactic transformation of the cubic-spinel to hexagonal-corundum structure. The textured sample permits us to obtain information on the spin reorientation behavior of the pressure transformed hematite in compression and decompression sequences. Spin reorientation is restricted to ∼15° over wide pressure ranges, attributable to the effect of entrapped vacancies in the high pressure structure. Thus there are structural and magnetic peculiarities specific to pressure transformed hematite not evident in pressurized hematite starting material. These are triggered by the maghemite→hematite transformation. - Graphical abstract: Pressure instigated topotactic transformation of vacancy ordered γ-Fe 2 O 3 →α-Fe 2 O 3 . There is restricted spin (B hf ) reorientation in the new pressure transformed hematite due to entrapped vacancies. The change in direction of V zz signifies a distortion of the FeO 6 octahedral local environment. Highlights: ► Robust vacancy ordered superstructure in maghemite to high pressures. ► Pressure instigated topotactic transformation to hematite and subsequent texture. ► Defect trapping in the pressure transformed hematite. ► Entrapped defects restricts spin reorientation in pressure transformed hematite. ► Contrasting behavior with pressurized hematite starting material.

Electron spin exchange of shallow donor muonium states

International Nuclear Information System (INIS)

Senba, Masayoshi

2005-01-01

Shallow donor muonium states with small hyperfine frequencies, recently observed in II-VI semiconductor compounds, have a number of unique features that present both opportunities and challenges in understanding muon spin dynamics in the presence of Heisenberg spin exchange. First, the shallow muonium state in CdSe with hyperfine frequency ω 0 /2π ∼ 0.1 MHz is already in the high field regime even in the earth's magnetic field, where only two precession frequencies are observable by the muon spin rotation (μSR) technique. Second, unlike in the case of more conventional muonium species with a larger hyperfine frequency, the μSR signal of shallow muonium states can be observed even in the transition region, between the slow spin-flip regime and the fast spin-flip regime, where the spin-flip rate and the hyperfine frequency are comparable. The muon spin dynamics in the transition region has not been theoretically explored previously, mainly because normal muonium in vacuum gives no observable signal in this region. Third, in the case of shallow muonium states, the incoherent process defined to be those spin-flip collisions that cause changes in muon spin precession frequencies, becomes crucially important in the transition region, where the incoherent process is entirely negligible in more conventional muonium species. By taking incoherent multiple collisions into account, an analytical expression for the time evolution of the muon spin polarization in Mu is derived, where Mu undergoes repeated spin-flip collisions. Comparisons with Monte Carlo calculations show that the analytical expression obtained in this work can reliably be used to analyse experimental data for shallow donor states not only in the slow spin-flip regime, but also in the transition region up to the onset of the fast regime. The present work confirms a recent experimental finding that, in the transition region, the initial phases of the two precession components of shallow donor states

Structural basis of lipid-driven conformational transitions in the KvAP voltage-sensing domain.

Science.gov (United States)

Li, Qufei; Wanderling, Sherry; Sompornpisut, Pornthep; Perozo, Eduardo

2014-02-01

Voltage-gated ion channels respond to transmembrane electric fields through reorientations of the positively charged S4 helix within the voltage-sensing domain (VSD). Despite a wealth of structural and functional data, the details of this conformational change remain controversial. Recent electrophysiological evidence showed that equilibrium between the resting ('down') and activated ('up') conformations of the KvAP VSD from Aeropyrum pernix can be biased through reconstitution in lipids with or without phosphate groups. We investigated the structural transition between these functional states, using site-directed spin-labeling and EPR spectroscopic methods. Solvent accessibility and interhelical distance determinations suggest that KvAP gates through S4 movements involving an ∼3-Å upward tilt and simultaneous ∼2-Å axial shift. This motion leads to large accessibly changes in the intracellular water-filled crevice and supports a new model of gating that combines structural rearrangements and electric-field remodeling.

Effect of spin structure transition in IrMn on the CoPd/IrMn perpendicular exchange biased system

Energy Technology Data Exchange (ETDEWEB)

Janjua, Muhammad Bilal; Guentherodt, Gernot [II. Physikalisches Institut A, RWTH Aachen University, Aachen (Germany)

2011-07-01

The exchange bias (EB) phenomenon is studied in MBE grown Pd(10 nm)/CoPd(x=8,16,30 nm)/IrMn(15 nm)/Pd(4 nm) samples, which exhibit a perpendicular anisotropy of Co22Pd78. These samples are field cooled along the out-of-plane direction and hysteresis loops are measured along both the out-of-plane and in-plane directions. It is observed that there is a transition temperature where the out-of-plane EB becomes greater than the in-plane EB. This behavior of EB is an evidence of the change in the spin structure of the given system, which is also revealed by the magnetization versus temperature measurements of the exchange biased and of the sole IrMn samples. It is found that with increasing temperature there is a spin structure transition in Ir25Mn75 (15nm) related to the 2Q to 3Q transition in the bulk, which is responsible for the increase in out-of-plane EB. A vertical shift in the hysteresis loop is also observed in these exchange biased samples at low temperatures (T<50 K).

Exact phase boundaries and topological phase transitions of the X Y Z spin chain

Science.gov (United States)

Jafari, S. A.

2017-07-01

Within the block spin renormalization group, we give a very simple derivation of the exact phase boundaries of the X Y Z spin chain. First, we identify the Ising order along x ̂ or y ̂ as attractive renormalization group fixed points of the Kitaev chain. Then, in a global phase space composed of the anisotropy λ of the X Y interaction and the coupling Δ of the Δ σzσz interaction, we find that the above fixed points remain attractive in the two-dimesional parameter space. We therefore classify the gapped phases of the X Y Z spin chain as: (1) either attracted to the Ising limit of the Kitaev-chain, which in turn is characterized by winding number ±1 , depending on whether the Ising order parameter is along x ̂ or y ̂ directions; or (2) attracted to the charge density wave (CDW) phases of the underlying Jordan-Wigner fermions, which is characterized by zero winding number. We therefore establish that the exact phase boundaries of the X Y Z model in Baxter's solution indeed correspond to topological phase transitions. The topological nature of the phase transitions of the X Y Z model justifies why our analytical solution of the three-site problem that is at the core of the present renormalization group treatment is able to produce the exact phase boundaries of Baxter's solution. We argue that the distribution of the winding numbers between the three Ising phases is a matter of choice of the coordinate system, and therefore the CDW-Ising phase is entitled to host appropriate form of zero modes. We further observe that in the Kitaev-chain the renormalization group flow can be cast into a geometric progression of a properly identified parameter. We show that this new parameter is actually the size of the (Majorana) zero modes.

Ferromagnetism and spin glass ordering in transition metal alloys (invited)

Science.gov (United States)

Crane, S.; Carnegie, D. W., Jr.; Claus, H.

1982-03-01

Magnetic properties of transition metal alloys near the percolation threshold are often complicated by metallurgical effects. Alloys like AuFe, VFe, CuNi, RhNi, and PdNi are in general not random solid solutions but have various degrees of atomic clustering or short-range order (SRO), depending on the heat treatment. First, it is shown how the magnetic ordering temperature of these alloys varies with the degree of clustering or SRO. Second, by systematically changing this degree of clustering or SRO, important information can be obtained about the magnetic phase diagram. In all these alloys below the percolation limit, the onset of ferromagnetic order is probably preceded by a spin glass-type ordering. However, details of the magnetic phase diagram near the critical point can be quite different alloy systems.

Quantum-Classical Phase Transition of the Escape Rate of Two-Sublattice Antiferromagnetic Large Spins

Science.gov (United States)

Owerre, Solomon Akaraka; Paranjape, M. B.

2014-11-01

The Hamiltonian of a two-sublattice antiferromagnetic spins, with single (hard-axis) and double ion anisotropies described by H = J {\\hat S}1...\\hatS 2-2Jz \\hat {S}1z\\hat {S}2z+K(\\hat {S}1z2 +\\hat {S}2z2) is investigated using the method of effective potential. The problem is mapped to a single particle quantum-mechanical Hamiltonian in terms of the relative coordinate and reduced mass. We study the quantum-classical phase transition of the escape rate of this model. We show that the first-order phase transition for this model sets in at the critical value Jc = (Kc+Jz, c)/2 while for the anisotropic Heisenberg coupling H = J(S1xS2x +S1yS2y) + JzS1zS2z + K(S1z2+ S2z2) we obtain Jc = (2Kc-Jz, c)/3. The phase diagrams of the transition are also studied.

Topological phase transition in the quench dynamics of a one-dimensional Fermi gas with spin-orbit coupling

Science.gov (United States)

Wang, Pei; Yi, Wei; Xianlong, Gao

2015-01-01

We study the quench dynamics of a one-dimensional ultracold Fermi gas with synthetic spin-orbit coupling. At equilibrium, the ground state of the system can undergo a topological phase transition and become a topological superfluid with Majorana edge states. As the interaction is quenched near the topological phase boundary, we identify an interesting dynamical phase transition of the quenched state in the long-time limit, characterized by an abrupt change of the pairing gap at a critical quenched interaction strength. We further demonstrate the topological nature of this dynamical phase transition from edge-state analysis of the quenched states. Our findings provide interesting clues for the understanding of topological phase transitions in dynamical processes, and can be useful for the dynamical detection of Majorana edge states in corresponding systems.

Some recent developments in spin glasses

Indian Academy of Sciences (India)

I give some experimental and theoretical background to spin glasses, and then discuss the nature of the phase transition in spin glasses with vector spins. Results of Monte Carlo simulations of the Heisenberg spin glass model in three dimensions are presented. A finite-size scaling analysis of the correlation length of the ...

Spin-flip tunneling in quantum dots

Energy Technology Data Exchange (ETDEWEB)

Schreiber, Lars; Braakman, Floris; Meunier, Tristan; Calado, Victor; Vandersypen, Lieven [Kavli Institute of NanoScience, Delft (Netherlands); Wegscheider, Werner [Institute for Experimental and Applied Physics, University of Regensburg (Germany)

2010-07-01

Electron spins in a gate-defined double quantum dot formed in a GaAs/(Al,Ga)As 2DEG are promising candidates for quantum information processing as coherent single spin rotation and spin swap has been demonstrated recently. In this system we investigate the two-electron spin dynamics in the presence of microwaves (5.20 GHz) applied to one side gate. During microwave excitation we observe characteristic photon assisted tunneling (PAT) peaks at the (1,1) to (0,2) charge transition. Some of the PAT peaks are attributed to photon tunneling events between the singlet S(0,2) and the singlet S(1,1) states, a spin-conserving transition. Surprisingly, other PAT peaks stand out by their different external magnetic field dependence. They correspond to tunneling involving a spin-flip, from the (0,2) singlet to a (1,1) triplet. The full spectrum of the observed PAT lines is captured by simulations. This process offers novel possibilities for 2-electron spin manipulation and read-out.

Efficient spin transitions in inelastic electron tunneling spectroscopy.

Science.gov (United States)

Lorente, Nicolás; Gauyacq, Jean-Pierre

2009-10-23

The excitation of the spin degrees of freedom of an adsorbed atom by tunneling electrons is computed using strong coupling theory. Recent measurements [Heinrich, Science 306, 466 (2004)] reveal that electron currents in a magnetic system efficiently excite its magnetic moments. Our theory shows that the incoming electron spin strongly couples with that of the adsorbate so that memory of the initial spin state is lost, leading to large excitation efficiencies. First-principles transmissions are evaluated in quantitative agreement with the experiment.

A geometrical approach to determine reorientation start and continuation conditions in ferromagnetic shape memory alloys considering the effects of loading history

International Nuclear Information System (INIS)

Shirani, M; Kadkhodaei, M

2014-01-01

Ferromagnetic shape memory alloys (FSMAs) and magnetic shape memory alloys (MSMAs) are metallic alloys that can undergo inelastic responses when exposed to magnetic fields. Several constitutive models have been proposed so far to model the behaviors of FSMAs. In this work, the effects of loading history on reorientation start conditions are considered, and it is shown that reorientation start conditions are not fixed values; rather, they change with respect to the amount of loading history. To consider the effects of loading history on reorientation start conditions, an available phase diagram in stress-field space is generalized to reorientation surfaces in stress-field-loading history space. Correspondingly, kinetic laws are derived in a continuum framework to be used with the reorientation surfaces to determine the amount of the martensitic variant 2 volume fraction. Based on the geometry of the reorientation surfaces, conditions that must be satisfied to ensure the continuation of reorientations are obtained. Available experimental findings validate the proposed model and the reorientation surfaces. (paper)

Control over the magnetism and transition between high- and low-spin states of an adatom on trilayer graphene.

Science.gov (United States)

Zheng, Anmin; Gao, Guoying; Huang, Hai; Gao, Jinhua; Yao, Kailun

2017-05-31

Using density-functional theory, we investigate the electronic and magnetic properties of an adatom (Na, Cu and Fe) on ABA- and ABC-stacked (Bernal and rhombohedral) trilayer graphenes. In particular, we study the influence of an applied gate voltage on magnetism, as it modifies the electronic states of the trilayer graphene (TLG) as well as changes the adatom spin states. Our study performed for a choice of three different adatoms (Na, Cu, and Fe) shows that the nature of adatom-graphene bonding evolves from ionic to covalent in moving from an alkali metal (Na) to a transition metal (Cu or Fe). Applying an external electric field (EEF) to TLG systems with different stacking orders results in the transition between high- and low-spin states in the latter case (Cu, Fe) and induces a little of magnetism in the former (Na) without magnetism in the absence of an external electric field. Our study would be useful for controlled adatom magnetism and (organic) spintronic applications in nanotechnology.

Spontaneous spin polarization in quantum wires

Energy Technology Data Exchange (ETDEWEB)

Vasilchenko, A.A., E-mail: a_vas2002@mail.ru

2015-12-04

The total energy of a quasi-one-dimensional electron system was calculated using the density functional theory. In the absence of a magnetic field, we have found that ferromagnetic state occurs in the quantum wires. The phase diagram of the transition into the spin-polarized state is constructed. The critical electron density below which electrons are in spin-polarized state is estimated analytically. - Highlights: • Density functional theory used to study a spin-polarized state in quantum wires. • The Kohn–Sham equation for quasi-one-dimensional electrons solved numerically. • The phase diagram of the transition into the spin-polarized state is constructed. • The electron density below which electrons are in a spin-polarized state was found. • The critical density of electrons was estimated analytically.

Spontaneous spin polarization in quantum wires

International Nuclear Information System (INIS)

Vasilchenko, A.A.

2015-01-01

The total energy of a quasi-one-dimensional electron system was calculated using the density functional theory. In the absence of a magnetic field, we have found that ferromagnetic state occurs in the quantum wires. The phase diagram of the transition into the spin-polarized state is constructed. The critical electron density below which electrons are in spin-polarized state is estimated analytically. - Highlights: • Density functional theory used to study a spin-polarized state in quantum wires. • The Kohn–Sham equation for quasi-one-dimensional electrons solved numerically. • The phase diagram of the transition into the spin-polarized state is constructed. • The electron density below which electrons are in a spin-polarized state was found. • The critical density of electrons was estimated analytically.

Language and Spatial Reorientation: Evidence from Severe Aphasia

Science.gov (United States)

Bek, Judith; Blades, Mark; Siegal, Michael; Varley, Rosemary

2010-01-01

Investigating spatial cognition in individuals with acquired language impairments can inform our understanding of how components of language are involved in spatial representation. Using the reorientation paradigm of Hermer-Vazquez, Spelke, and Katsnelson (1999), we examined spatial cue integration (landmark-geometry conjunctions) in individuals…

Distribution of spin dipole transition strength in the 15N(n,p)15C reaction

International Nuclear Information System (INIS)

Cellar, A.; Alford, W.P.; Helmer, R.; Abegg, R.; Frekers, D.; Haeusser, O.; Henderson, R.S.; Jackson, K.P.; Vetterli, M.; Yen, S.; Jeppesen, R.; Larson, B.; Mildenberger, J.; Pointon, B.W.; Trudel, A.

1990-08-01

The reaction 15 N(n,p) 15 C was studied at a neutron energy of 288 MeV using the TRIUMF (n,p) charge exchange facility and a high pressure gas target. The angular distributions for spin dipole (ΔL=1) transitions to the states in 15 C at energies 0 MeV and 0.740 MeV, as well as for higher excitation energies, were measured and the results were compared with DWIA calculations. The measured distribution of the spin dipole strength agrees well with shell model predictions, indicating that a rather simple model provides a satisfactory description of the 15 N ground state, and of positive parity states in 15 C up to about 18 MeV excitation. The magnitude of the peak cross sections (at ≅ 7 degrees) is described well by the calculations when the theoretical cross section is renormalized by a factor 0.7. The calculated cross sections near zero degrees are generally smaller than experimental data. It this is a general feature of ΔL=1 transitions, it suggests that estimates of GT strength based on a multipole decomposition of measured cross sections may be too high. (Author) (41 refs., 3 tabs., 14 figs.)

Micromagnetic analysis of spin-reorientation transitions. The role of magnetic domain structure

Energy Technology Data Exchange (ETDEWEB)

Skokov, Konstantin P., E-mail: skokov_k_p@mail.ru [Tver State University, Tver 170100 (Russian Federation); Physics Department, Chelyabinsk State University, Chelyabinsk 454001 (Russian Federation); Pastushenkov, Yury G., E-mail: yupast@mail.ru [Tver State University, Tver 170100 (Russian Federation); Taskaev, Sergey V., E-mail: tsv@csu.ru [Physics Department, Chelyabinsk State University, Chelyabinsk 454001 (Russian Federation); National University of Science and Technology “MISiS”, Moscow 119049 (Russian Federation); Rodionova, Valeria V., E-mail: valeriarodionova@gmail.com [National University of Science and Technology “MISiS”, Moscow 119049 (Russian Federation); Immanuel Kant Baltic Federal University, Kaliningrad 236041 (Russian Federation)

2015-12-01

A method for calculating micromagnetic state of ferro- or ferrimagnetic single-crystals based on the Néel's method of phases is proposed. The standard Néel technique requires different approaches to calculation of micromagnetic state of samples with different anisotropy types. Furthermore, this technique cannot be used to calculate magnetization curves of materials with a complex anisotropy type, in which the first-order magnetization process (FOMP) occurs. On the contrary, the technique proposed in the present work makes it possible to calculate micromagnetic state of a sample within one unified approach. This technique has no limitations in terms of the anisotropy type as well. In case of the FOMP, the simulation methods that we used show results different from conventional calculation methods. The reason is that the conventional methods imply coherent rotation of magnetization in single domain particle (so-called Stoner–Wohlfarth model). We explain this discrepancy by the fact that a magnetic domain structure appears in the region of the FOMP. In the present work we show that magnetization processes do not occur in a jump under the FOMP but gradually pass though nucleation and new high-field phase growing, which substitutes for the low-field phase.

Micromagnetic analysis of spin-reorientation transitions. The role of magnetic domain structure

International Nuclear Information System (INIS)

Skokov, Konstantin P.; Pastushenkov, Yury G.; Taskaev, Sergey V.; Rodionova, Valeria V.

2015-01-01

A method for calculating micromagnetic state of ferro- or ferrimagnetic single-crystals based on the Néel's method of phases is proposed. The standard Néel technique requires different approaches to calculation of micromagnetic state of samples with different anisotropy types. Furthermore, this technique cannot be used to calculate magnetization curves of materials with a complex anisotropy type, in which the first-order magnetization process (FOMP) occurs. On the contrary, the technique proposed in the present work makes it possible to calculate micromagnetic state of a sample within one unified approach. This technique has no limitations in terms of the anisotropy type as well. In case of the FOMP, the simulation methods that we used show results different from conventional calculation methods. The reason is that the conventional methods imply coherent rotation of magnetization in single domain particle (so-called Stoner–Wohlfarth model). We explain this discrepancy by the fact that a magnetic domain structure appears in the region of the FOMP. In the present work we show that magnetization processes do not occur in a jump under the FOMP but gradually pass though nucleation and new high-field phase growing, which substitutes for the low-field phase.

Detection of individual spin transitions of a single proton confined in a cryogenic Penning trap

Energy Technology Data Exchange (ETDEWEB)

Kracke, Holger

2013-02-27

The presented experiment for the determination of the magnetic moment of the proton is based on the measurement of the ratio of cyclotron frequency and Larmor frequency of a single proton confined in a cryogenic double-Penning trap. In the course of this thesis, the simultaneous non-destructive measurement of two of the three eigenfrequencies of the proton in thermal equilibrium with corresponding detection systems was demonstrated, which reduces the measurement time of the cyclotron frequency by a factor of two. Furthermore, this thesis presents the first detection of individual spin transitions of a single proton, which allows for the determination of the Larmor frequency. The continuous Stern-Gerlach effect is utilized to couple the magnetic moment to the axial mode of the trapped proton by means of a magnetic bottle. Thus, a spin flip causes a jump of the axial frequency, which can be measured non-destructively with highly-sensitive detection systems. However, not only the spin momentum is coupled to the axial motion but also the angular momentum. Thus, the main experimental challenge is the elimination of energy fluctuations in the radial modes in order to maintain spin flip resolution. Due to systematic studies on the stability of the axial frequency and a complete revision of the experimental setup, this goal was achieved. The spin state of the proton can be determined with very high fidelity for the very first time. Thus, this thesis represents an important step towards a high-precision determination of the magnetic moment of the proton.

Spin Flips versus Spin Transport in Nonthermal Electrons Excited by Ultrashort Optical Pulses in Transition Metals

Science.gov (United States)

Shokeen, V.; Sanchez Piaia, M.; Bigot, J.-Y.; Müller, T.; Elliott, P.; Dewhurst, J. K.; Sharma, S.; Gross, E. K. U.

2017-09-01

A joint theoretical and experimental investigation is performed to understand the underlying physics of laser-induced demagnetization in Ni and Co films with varying thicknesses excited by 10 fs optical pulses. Experimentally, the dynamics of spins is studied by determining the time-dependent amplitude of the Voigt vector, retrieved from a full set of magnetic and nonmagnetic quantities performed on both sides of films, with absolute time reference. Theoretically, ab initio calculations are performed using time-dependent density functional theory. Overall, we demonstrate that spin-orbit induced spin flips are the most significant contributors with superdiffusive spin transport, which assumes only that the transport of majority spins without spin flips induced by scattering does not apply in Ni. In Co it plays a significant role during the first ˜20 fs only. Our study highlights the material dependent nature of the demagnetization during the process of thermalization of nonequilibrium spins.

Quantum spin Hall effect and topological phase transition in InN x Bi y Sb1-x-y /InSb quantum wells

Science.gov (United States)

Song, Zhigang; Bose, Sumanta; Fan, Weijun; Zhang, Dao Hua; Zhang, Yan Yang; Shen Li, Shu

2017-07-01

Quantum spin Hall (QSH) effect, a fundamentally new quantum state of matter and topological phase transitions are characteristics of a kind of electronic material, popularly referred to as topological insulators (TIs). TIs are similar to ordinary insulator in terms of their bulk bandgap, but have gapless conducting edge-states that are topologically protected. These edge-states are facilitated by the time-reversal symmetry and they are robust against nonmagnetic impurity scattering. Recently, the quest for new materials exhibiting non-trivial topological state of matter has been of great research interest, as TIs find applications in new electronics and spintronics and quantum-computing devices. Here, we propose and demonstrate as a proof-of-concept that QSH effect and topological phase transitions can be realized in {{InN}}x{{Bi}}y{{Sb}}1-x-y/InSb semiconductor quantum wells (QWs). The simultaneous incorporation of nitrogen and bismuth in InSb is instrumental in lowering the bandgap, while inducing opposite kinds of strain to attain a near-lattice-matching conducive for lattice growth. Phase diagram for bandgap shows that as we increase the QW thickness, at a critical thickness, the electronic bandstructure switches from a normal to an inverted type. We confirm that such transition are topological phase transitions between a traditional insulator and a TI exhibiting QSH effect—by demonstrating the topologically protected edge-states using the bandstructure, edge-localized distribution of the wavefunctions and edge-state spin-momentum locking phenomenon, presence of non-zero conductance in spite of the Fermi energy lying in the bandgap window, crossover points of Landau levels in the zero-mode indicating topological band inversion in the absence of any magnetic field and presence of large Rashba spin-splitting, which is essential for spin-manipulation in TIs.

High-spin states in the transitional odd-odd nuclei 150Eu and 152Tb

International Nuclear Information System (INIS)

Barneoud, D.; Foin, C.; Pinston, J.A.; Monnand, E.

1983-06-01

The ( 7 Li, 5n) and ( 11 B, 5n) reactions have been used to study the high-spin states in the two odd-odd nuclei 150 Eu and 152 Tb. Three decoupled bands have been evidenced in each nucleus belonging to the same configurations [f 7/2]sub(n) [h 11/2]sub(p), [h 9/2]sub(n) [h 11/2 ]sub(p) and [i 13/2]sub(n) [h 11/2]sub(p). The latter one is well developped and improves our knowledge of this system between the spherical and deformed region. The analysis of the collective moment of inertia and transition ratios strongly suggests an increase of the deformation when the rotational frequency increases in these two transitional nuclei 150 Eu and 152 Tb

Electron Spin Resonance Studies of Carbonic Anhydrase: Transition Metal Ions and Spin-Labeled Sulfonamides*

Science.gov (United States)

Taylor, June S.; Mushak, Paul; Coleman, Joseph E.

1970-01-01

Electron spin resonance (esr) spectra of Cu(II) and Co(II) carbonic anhydrase, and a spin-labeled sulfonamide complex of the Zn(II) enzyme, are reported. The coordination geometry of Cu(II) bound in the enzyme appears to have approximately axial symmetry. Esr spectra of enzyme complexes with metal-binding anions also show axial symmetry and greater covalency, in the order ethoxzolamide cyanide complex suggests the presence of two, and probably three, equivalent nitrogen ligands from the protein. Esr spectra of the Co(II) enzyme and its complexes show two types of Co(II) environment, one typical of the native enzyme and the 1:1 CN- complex, and one typical of a 2:1 CN- complex. Co(II) in the 2:1 complex appears to be low-spin and probably has a coordination number of 5. Binding of a spin-labeled sulfonamide to the active center immobilizes the free radical. The similarity of the esr spectra of spin-labeled Zn(II) and Co(II) carbonic anhydrases suggests that the conformation at the active center is similar in the two metal derivatives. PMID:4320976

Educating Academic Staff to Reorient Curricula in ESD

Science.gov (United States)

Biasutti, Michele; Makrakis, Vassilios; Concina, Eleonora; Frate, Sara

2018-01-01

Purpose: The purpose of this paper is to present a professional development experience for higher education academic staff within the framework of an international Tempus project focused on reorienting university curricula to address sustainability. The project included revising curricula to phase sustainable development principles into university…

Stochastic kinetics of photoinduced phase transitions in spin-crossover solids

Science.gov (United States)

Gudyma, Iurii; Maksymov, Artur; Dimian, Mihai

2013-10-01

We study the stochastic macroscopic kinetics of photoinduced phase transitions in spin-crossover compounds assisted by white and colored Ornstein-Uhlenbeck noise. By using a phenomenological master equation obtained in the mean-field approach, the phase diagram is constructed based on the associated Lyapunov function. The stochastic behavior is then analyzed in the Langevin framework and the corresponding Fokker-Planck equations. Both additive and multiplicative and white and colored types of noise are considered and the stationary probability densities are found along with the noise-assisted light induced hysteretic loops. By using the Kramers formalism, we also focus our attention on the escape time problem in these noise perturbed systems. A detailed study of the relative escape time dependence on various noise characteristics is performed and the main features are compared for different types of noise.

Quantum phase transitions in spin-1 X X Z chains with rhombic single-ion anisotropy

Science.gov (United States)

Ren, Jie; Wang, Yimin; You, Wen-Long

2018-04-01

We explore numerically the inverse participation ratios in the ground state of one-dimensional spin-1 X X Z chains with the rhombic single-ion anisotropy. By employing the techniques of density-matrix renormalization group, effects of the rhombic single-ion anisotropy on various information theoretical measures are investigated, such as the fidelity susceptibility, the quantum coherence, and the entanglement entropy. Their relations with the quantum phase transitions are also analyzed. The phase transitions from the Y -Néel phase to the large-Ex or the Haldane phase can be well characterized by the fidelity susceptibility. The second-order derivative of the ground-state energy indicates all the transitions are of second order. We also find that the quantum coherence, the entanglement entropy, the Schmidt gap, and the inverse participation ratios can be used to detect the critical points of quantum phase transitions. Results drawn from these quantum information observables agree well with each other. Finally we provide a ground-state phase diagram as functions of the exchange anisotropy Δ and the rhombic single-ion anisotropy E .

Modulation Algorithms for Manipulating Nuclear Spin States

OpenAIRE

Liu, Boyang; Zhang, Ming; Dai, Hong-Yi

2013-01-01

We exploit the impact of exact frequency modulation on transition time of steering nuclear spin states from theoretical point of view. 1-stage and 2-stage Frequency-Amplitude-Phase modulation (FAPM) algorithms are proposed in contrast with 1-stage and 3-stage Amplitude-Phase modulation (APM) algorithms. The sufficient conditions are further present for transiting nuclear spin states within the specified time by these four modulation algorithms. It is demonstrated that transition time performa...

Spin-State Transition in La1-xSrxCoO3 Single Crystals

Science.gov (United States)

Bhardwaj, S.; Prabhakaran, D.; Awasthi, A. M.

2011-07-01

We present a study of the thermal conductivity (κ), specific heat (Cp) and Raman spectra of La1-xSrxCoO3 (x = 0,0.1) single crystals. Both the specimens have low thermal conductivity and board Raman peaks, arising from strong scattering of phonons by lattice disorder, produced by (and doping-enhanced) spin-states admixture of the Co3+ ions. The thermal conductivity anomalously deviates from ˜1/T behaviour at high (room) temperatures, expected of an insulator. High-temperature specific heat reveals large decrease in the metal-insulator (M-I) transition temperature with Sr-doping.

Irreversibility and self-organization in spin glasses. 1. Origin of irreversibility in spin glasses

International Nuclear Information System (INIS)

Kovrov, V.P.; Kurbatov, A.M.

1989-05-01

The origin of irreversibility in spin glasses is found out on the basis of the analytical study of the well-known TAP equations. Connection between irreversible jumpwise transitions and a positive feedback in spin glasses is discussed. (author). 7 refs, 4 figs

Spin reorientation behavior in Yb doped YMnO3

International Nuclear Information System (INIS)

Sharma, Neetika; Das, A.

2014-01-01

RMnO 3 with smaller rare-earths ions (R = Ho to Lu and Y) crystallize in the non-centrosymmetric hexagonal space group P6 3 cm. The magnetic structure of RMnO 3 compounds with (R=Er,Yb.Lu) are described by irreducible representations (IR) Γ 2,4 and Γ 1,3 for those with higher ionic radii (R=Ho,Y,Y-Er). Of recent the magnetic structure of YMnO 3 has been found to be better described by Γ 3 + Γ 4 IR. YbMnO 3 is another hexagonal manganite, with almost similar transition temperature, and basically shares all the physical properties of YMnO 3 , except for the magnetic structure. The magnetic structure of YbMnO 3 can be explained by Γ 2 or Γ 4 . The non collinear nature of magnetic ordering in these compounds arises due to the frustration inherent in these compounds. In this study we have probed the effect of a magnetic ion (Yb) on the magnetic structure of these frustrated isostructural compounds

Spin reorientation in HoIG investigated by means of Faraday effect

International Nuclear Information System (INIS)

Balanda, M.; Niziol, S.

1979-01-01

Faraday rotation measurements in pulsed magnetic fields up to 160 kOe and in low dc fields are carried out for Ho 3 Fe 5 O 12 near the compensation point. Transition to the canted phase is observed and the temperature dependence of the critical field determined. From the holmium sublattice magnetization and Hsub(cr) versus. T gradient, values of the two molecular field coefficients are determined. (author)

A signature for isoscalar-spin transitions in (d vector, d' vector) scattering at intermediate energy

International Nuclear Information System (INIS)

Morlet, M.; Bimbot, L.; Guillot, J.; Johnson, B.N.; Jourdan, F.; Langevin-Joliot, H.; Marty, N.; Rosier, L.; Wiele, J. van de; Willis, A.; Beatty, D.; Edwards, G.; Fergerson, R.W.; Glashausser, C.; Green, A.; Djalali, C.; Johnson, B.N.; Tomasi-Gustafsson, E.; Youn, M.Y.

1991-05-01

Three different signatures for isoscalar spin transitions in nuclei have been tested in the 12 C(d,d') 12 C reaction at 400 MeV. These signatures have values close to zero for the natural parity states, and range from 0.22 to 0.50 for the ΔS=1 ΔT=0, 12.7 MeV state. Preliminary results on 40 Ca(d,d') at 400 MeV are also presented. (author) 26 refs., 4 figs., 1 tab

Manipulation of the spin in single molecule magnets via Landau-Zener transitions

Science.gov (United States)

Palii, Andrew; Tsukerblat, Boris; Clemente-Juan, Juan M.; Gaita-Ariño, Alejandro; Coronado, Eugenio

2011-11-01

We theoretically investigate the effects of a magnetic pulse on a single-molecule magnet (SMM) initially magnetized by a dc field along the easy axis of magnetization. In the Landau-Zener (LZ) scheme, it is shown that the final spin state is a function of the shape and duration of the pulse, conditioned by the decoherence time of the SMM. In the case of coherent tunneling, the asymmetric pulses are shown to reverse the direction of the magnetization, while the symmetric pulses can only decrease the value of the initial magnetization. It is also demonstrated that the application of an external variable dc field in the hard plane of magnetization provides the possibility to tune the resulting magnetization due to quantum interference effects. The results and the conditions for the observation of the pulse-triggered LZ transitions are illustrated by the application of the proposed scheme to the well-studied single-molecule magnet Fe8. To put the results into perspective, some potential applications of SMMs experiencing pulse-induced LZ transitions, such as switching devices and qubits, are discussed.

Pressure response of vacancy ordered maghemite ({gamma}-Fe{sub 2}O{sub 3}) and high pressure transformed hematite ({alpha}-Fe{sub 2}O{sub 3})

Energy Technology Data Exchange (ETDEWEB)

Hearne, Giovanni, E-mail: grhearne@uj.ac.za [Department of Physics, University of Johannesburg, PO Box 524, Auckland Park, 2006 Johannesburg (South Africa); Pischedda, Vittoria, E-mail: Vittoria.Pischedda@univ-lyon1.fr [Laboratoire de Physique de la Matiere Condensee et Nanostructures, University Lyon 1 and CNRS, 69622 Villeurbanne Cedex (France)

2012-03-15

Combined XRD and Moessbauer effect spectroscopy studies to high pressures of {approx}30 GPa of vacancy ordered maghemite are presented. The vacancy ordered superstructure is robust and remains intact up to the pressure-induced onset transition to hematite at 13-16 GPa. The pressure transformed hematite is shown to be crystallographically textured, unlike the randomised low pressure maghemite phase. This arises out of a pressure or stress instigated topotactic transformation of the cubic-spinel to hexagonal-corundum structure. The textured sample permits us to obtain information on the spin reorientation behavior of the pressure transformed hematite in compression and decompression sequences. Spin reorientation is restricted to {approx}15 Degree-Sign over wide pressure ranges, attributable to the effect of entrapped vacancies in the high pressure structure. Thus there are structural and magnetic peculiarities specific to pressure transformed hematite not evident in pressurized hematite starting material. These are triggered by the maghemite{yields}hematite transformation. - Graphical abstract: Pressure instigated topotactic transformation of vacancy ordered {gamma}-Fe{sub 2}O{sub 3}{yields}{alpha}-Fe{sub 2}O{sub 3}. There is restricted spin (B{sub hf}) reorientation in the new pressure transformed hematite due to entrapped vacancies. The change in direction of V{sub zz} signifies a distortion of the FeO{sub 6} octahedral local environment. Highlights: Black-Right-Pointing-Pointer Robust vacancy ordered superstructure in maghemite to high pressures. Black-Right-Pointing-Pointer Pressure instigated topotactic transformation to hematite and subsequent texture. Black-Right-Pointing-Pointer Defect trapping in the pressure transformed hematite. Black-Right-Pointing-Pointer Entrapped defects restricts spin reorientation in pressure transformed hematite. Black-Right-Pointing-Pointer Contrasting behavior with pressurized hematite starting material.

Percolation and spin glass transition

International Nuclear Information System (INIS)

Sadiq, A.; Tahir-Kheli, R.A.; Wortis, M.; Bhatti, N.A.

1980-10-01

The behaviour of clusters of curved and normal plaquette particles in a bond random, +-J, Ising model is studied in finite square and triangular lattices. Computer results for the concentration of antiferromagnetic bonds when percolating clusters first appears are found to be close to those reported for the occurrence and disappearance of spin glass phases in these systems. (author)

Nano and micro reoriented domains and their relation with the crystal structure in the new ferroelectric boracite Zn3B7O13Br

International Nuclear Information System (INIS)

Campa-Molina, J; Ulloa-Godinez, S; Barrera, A; Bucio, L; Mata, J

2006-01-01

A new zinc brome boracite Zn 3 B 7 O 13 Br has been grown by a chemical transport reaction in closed quartz ampoules at 920 K. The crystal structure was characterized by Rietveld refinement. Ferroelectric nano and micro reorientable domains were found in this material using polarizing optical microscopy (PLM), scanning electron microscopy (SEM) and transmission electron microscopy (TEM). Chemical analysis was performed with x-ray energy dispersive spectroscopy (EDX). In the crystal, a new structure transition at 586 K from orthorhombic (Pca 2 1 ) to cubic cell (F4-bar3c) has been found. This transition was corroborated by differential scanning calorimetry (DSC)

Nano and micro reoriented domains and their relation with the crystal structure in the new ferroelectric boracite Zn3B7O13Br

Science.gov (United States)

Campa-Molina, J.; Ulloa-Godínez, S.; Barrera, A.; Bucio, L.; Mata, J.

2006-05-01

A new zinc brome boracite Zn3B7O13Br has been grown by a chemical transport reaction in closed quartz ampoules at 920 K. The crystal structure was characterized by Rietveld refinement. Ferroelectric nano and micro reorientable domains were found in this material using polarizing optical microscopy (PLM), scanning electron microscopy (SEM) and transmission electron microscopy (TEM). Chemical analysis was performed with x-ray energy dispersive spectroscopy (EDX). In the crystal, a new structure transition at 586 K from orthorhombic (Pca 21) to cubic cell (F\\overline 4 3c ) has been found. This transition was corroborated by differential scanning calorimetry (DSC).

A combined DFT and restricted open-shell configuration interaction method including spin-orbit coupling: Application to transition metal L-edge X-ray absorption spectroscopy

Energy Technology Data Exchange (ETDEWEB)

Roemelt, Michael; Maganas, Dimitrios; Neese, Frank [Max-Planck Institute for Chemical Energy Conversion, Stiftstrasse 34-36, D-45470 Muelheim an der Ruhr (Germany); DeBeer, Serena [Max-Planck Institute for Chemical Energy Conversion, Stiftstrasse 34-36, D-45470 Muelheim an der Ruhr (Germany); Department of Chemistry and Chemical Biology, Cornell University, Ithaca, New York 14853 (United States)

2013-05-28

A novel restricted-open-shell configuration interaction with singles (ROCIS) approach for the calculation of transition metal L-edge X-ray absorption spectra is introduced. In this method, one first calculates the ground state and a number of excited states of the non-relativistic Hamiltonian. By construction, the total spin is a good quantum number in each of these states. For a ground state with total spin S excited states with spin S Prime = S, S - 1, and S + 1 are constructed. Using Wigner-Eckart algebra, all magnetic sublevels with M{sub S}= S, Horizontal-Ellipsis , -S for each multiplet of spin S are obtained. The spin-orbit operator is represented by a mean-field approximation to the full Breit-Pauli spin-orbit operator and is diagonalized over this N-particle basis. This is equivalent to a quasi-degenerate treatment of the spin-orbit interaction to all orders. Importantly, the excitation space spans all of the molecular multiplets that arise from the atomic Russell-Saunders terms. Hence, the method represents a rigorous first-principles approach to the complicated low-symmetry molecular multiplet problem met in L-edge X-ray absorption spectroscopy. In order to gain computational efficiency, as well as additional accuracy, the excitation space is restricted to single excitations and the configuration interaction matrix is slightly parameterized in order to account for dynamic correlation effects in an average way. To this end, it is advantageous to employ Kohn-Sham rather than Hartree-Fock orbitals thus defining the density functional theory/ROCIS method. However, the method can also be used in an entirely non-empirical fashion. Only three global empirical parameters are introduced and have been determined here for future application of the method to any system containing any transition metal. The three parameters were carefully calibrated using the L-edge X-ray absorption spectroscopy spectra of a test set of coordination complexes containing first row

Spin Dynamics and Magnetic Ordering in Mixed Valence Systems

DEFF Research Database (Denmark)

Shapiro, S. M.; Bjerrum Møller, Hans; Axe, J. D.

1978-01-01

. 0 meV at the transition to the alpha phase. The temperature independence of the susceptibility within the gamma phase cannot be simply reconciled with the temperature dependence of the valence within the gamma phase. TmSe is shown to order in a type I antiferromagnetic structure below T//N similar 3....... 2 K. The magnetic phase diagram is understood as a successive domain reorientation and a metamagnetic phase transition for T less than 3 K with increasing field. The mixed valence nature manifests itself in a reduced moment and a markedly altered crystal field. Another sample of TmSe with a lattice...

Impact of silica environment on hyperfine interactions in ε-Fe.sub.2./sub.O.sub.3./sub. nanoparticles

Czech Academy of Sciences Publication Activity Database

Kubíčková, L.; Kohout, J.; Brázda, Petr; Veverka, Miroslav; Kmječ, T.; Kubániová, D.; Bezdička, Petr; Klementová, Mariana; Šantavá, Eva; Závěta, Karel

2016-01-01

Roč. 231, č. 1 (2016), s. 1-10, č. článku 159. ISSN 0304-3843 Institutional support: RVO:68378271 ; RVO:61388980 Keywords : iron oxide * polymorph of ferric oxide * 57 Fe Mössbauer spectrometry * ferrimagnetic nanoparticles * giant coercive field * spin-reorientation transition Subject RIV: BM - Solid Matter Physics ; Magnetism; CA - Inorganic Chemistry (UACH-T)

Transition from Spin Dewetting to continuous film in spin coating of Liquid Crystal 5CB.

Science.gov (United States)

Dhara, Palash; Bhandaru, Nandini; Das, Anuja; Mukherjee, Rabibrata

2018-05-08

Spin dewetting refers to spontaneous rupture of the dispensed solution layer during spin coating, resulting in isolated but periodic, regular sized domains of the solute and is pre-dominant when the solute concentration (C n ) is very low. In this article we report how the morphology of liquid crystal (LC) 5CB thin films coated on flat and patterned PMMA substrate transform from spin dewetted droplets to continuous films with increase in C n . We further show that within the spin dewetted regime, with gradual increase in the solute concentration, periodicity of the isotropic droplets (λ D ) as well as their mean diameter (d D ), gradually decreases, till the film becomes continuous at a critical concentration (C n *). Interestingly, the trend that λ D reduces with increase in C n is exact opposite to what is observed in thermal/solvent vapor induced dewetting of a thin film. The spin dewetted droplets exhibit transient Radial texture, in contrast to Schlieren texture observed in elongated threads and continuous films of 5CB, which remains in the Nematic phase at room temperature. Finally we show that by casting the film on a grating patterned substrate it becomes possible to align the spin dewetted droplets along the contours substrate patterns.

Spins of superdeformed rotational bands in Tl isotopes

Energy Technology Data Exchange (ETDEWEB)

Dadwal, Anshul; Mittal, H.M. [Dr. B.R. Ambedkar National Institute of Technology, Jalandhar (India)

2017-01-15

The two-parameter model defined for even-even nuclei viz. soft-rotor formula is used to assign the band-head spin of the 17 rotational bands in Tl isotopes. The least-squares fitting method is employed to obtain the spins of these bands in the A ∝ 190 mass region. The calculated transition energies are found to depend sensitively on the proposed spin. Whenever a correct spin assignment is made, the calculated and experimental transition energies coincide very well. The dynamic moment of inertia is also calculated and its variation with rotational frequency is explored. (orig.)

Coupled spin and charge collective excitations in a spin polarized electron gas

International Nuclear Information System (INIS)

Marinescu, D.C.; Quinn, J.J.; Yi, K.S.

1997-01-01

The charge and longitudinal spin responses induced in a spin polarized quantum well by a weak electromagnetic field are investigated within the framework of the linear response theory. The authors evaluate the excitation frequencies for the intra- and inter-subband transitions of the collective charge and longitudinal spin density oscillations including many-body corrections beyond the random phase approximation through the spin dependent local field factors, G σ ± (q,ω). An equation-of-motion method was used to obtain these corrections in the limit of long wavelengths, and the results are given in terms of the equilibrium pair correlation function. The finite degree of spin polarization is shown to introduce coupling between the charge and spin density modes, in contrast with the result for an unpolarized system

Low-temperature structural transition in the quasi-one-dimensional spin-1/2 compound L i2C u2O (SO4) 2

Science.gov (United States)

Rousse, G.; Rodríguez-Carvajal, J.; Giacobbe, C.; Sun, M.; Vaccarelli, O.; Radtke, G.

2017-04-01

A thorough structural exploration has been made on the quasi-one-dimensional S =1 /2 compound L i2C u2O (SO4) 2 by neutron and synchrotron x-ray diffraction. It reveals the occurrence of a structural transition at 125 K, characterized by a lowering of symmetry from P 42/m to P 1 ¯ , which is possibly driven by an exchange striction mechanism. This transition involves a dimerization of some Cu in the edge-sharing tetrahedral Cu chains. A symmetry mode analysis indicates that one representation, Γ3+Γ4+ , dominates the structural transition. Interestingly, no intermediate structure with P 112 /m symmetry is observed experimentally. Lastly, temperature dependent magnetic susceptibility measurements and neutron diffraction reveal that the magnetic ground state of this compound is a spin-singlet with a spin gap, characterized by the absence of long-range magnetic order down to 1.7 K.

Spin-orbit coupling and electric-dipole spin resonance in a nanowire double quantum dot.

Science.gov (United States)

Liu, Zhi-Hai; Li, Rui; Hu, Xuedong; You, J Q

2018-02-02

We study the electric-dipole transitions for a single electron in a double quantum dot located in a semiconductor nanowire. Enabled by spin-orbit coupling (SOC), electric-dipole spin resonance (EDSR) for such an electron can be generated via two mechanisms: the SOC-induced intradot pseudospin states mixing and the interdot spin-flipped tunneling. The EDSR frequency and strength are determined by these mechanisms together. For both mechanisms the electric-dipole transition rates are strongly dependent on the external magnetic field. Their competition can be revealed by increasing the magnetic field and/or the interdot distance for the double dot. To clarify whether the strong SOC significantly impact the electron state coherence, we also calculate relaxations from excited levels via phonon emission. We show that spin-flip relaxations can be effectively suppressed by the phonon bottleneck effect even at relatively low magnetic fields because of the very large g-factor of strong SOC materials such as InSb.

Reorientation response of magnetic microspheres attached to gold electrodes under an applied magnetic field

International Nuclear Information System (INIS)

De Los Santos Valladares, L.; Reeve, R.M.; Mitrelias, T.; Langford, R.M.; Barnes, C.H.W.; Bustamante Dominguez, A.; Aguiar, J. Albino; Majima, Y.

2013-01-01

In this work, we report the mechanical reorientation of thiolated ferromagnetic microspheres bridging a pair of gold electrodes under an external magnetic field. When an external magnetic field (7 kG) is applied during the measurement of the current-voltage characteristics of a carboxyl ferromagnetic microsphere (4 μm diameter) attached to two gold electrodes by self-assembled monolayers (SAMs) of octane dithiol (C 8 H 18 S 2 ), the current signal is distorted. Rather than due to magnetoresistance, this effect is caused by a mechanical reorientation of the ferromagnetic sphere, which alters the number of SAMs between the sphere and the electrodes and therefore affects conduction. To study the physical reorientation of the ferromagnetic particles, we measure their hysteresis loops while suspended in a liquid solution. (author)

Reorientation response of magnetic microspheres attached to gold electrodes under an applied magnetic field

Energy Technology Data Exchange (ETDEWEB)

De Los Santos Valladares, L.; Reeve, R.M.; Mitrelias, T.; Langford, R.M.; Barnes, C.H.W., E-mail: luis_d_v@hotmail.com [Cavendish Laboratory, Department of Physics, University of Cambridge Materials and Structures Laboratory (United Kingdom); Bustamante Dominguez, A. [Laboratorio de Ceramicos y Nanomateriales, Facultad de Ciencias Fisicas, Universidad Nacional Mayor de San Marcos, Lima (Peru); Aguiar, J. Albino [Universidade Federal de Pernambuco (UFPE), Recife, PE (Brazil). Departamento de Fisica; Azuma, Y. [Materials and Structures Laboratory, Tokyo Institute of Technology, Midori-ku, Yokohama (Japan); Majima, Y. [CREST, Japan Science and Technology Agency (JST), Midori-ku, Yokohama (Japan)

2013-08-15

In this work, we report the mechanical reorientation of thiolated ferromagnetic microspheres bridging a pair of gold electrodes under an external magnetic field. When an external magnetic field (7 kG) is applied during the measurement of the current-voltage characteristics of a carboxyl ferromagnetic microsphere (4 μm diameter) attached to two gold electrodes by self-assembled monolayers (SAMs) of octane dithiol (C{sub 8}H{sub 18}S{sub 2}), the current signal is distorted. Rather than due to magnetoresistance, this effect is caused by a mechanical reorientation of the ferromagnetic sphere, which alters the number of SAMs between the sphere and the electrodes and therefore affects conduction. To study the physical reorientation of the ferromagnetic particles, we measure their hysteresis loops while suspended in a liquid solution. (author)

INIST: databases reorientation

International Nuclear Information System (INIS)

Bidet, J.C.

1995-01-01

INIST is a CNRS (Centre National de la Recherche Scientifique) laboratory devoted to the treatment of scientific and technical informations and to the management of these informations compiled in a database. Reorientation of the database content has been proposed in 1994 to increase the transfer of research towards enterprises and services, to develop more automatized accesses to the informations, and to create a quality assurance plan. The catalog of publications comprises 5800 periodical titles (1300 for fundamental research and 4500 for applied research). A science and technology multi-thematic database will be created in 1995 for the retrieval of applied and technical informations. ''Grey literature'' (reports, thesis, proceedings..) and human and social sciences data will be added to the base by the use of informations selected in the existing GRISELI and Francis databases. Strong modifications are also planned in the thematic cover of Earth sciences and will considerably reduce the geological information content. (J.S.). 1 tab

Molecular reorientations in the nematic and rotatory phases of di-n-pentyloxyazoxybenzene

International Nuclear Information System (INIS)

Nguyen, X.P.; Krawczyk, J.; Chrusciel, D.

1986-04-01

Results of dielectric relaxation (DR), quasielastic neutron scattering (QNS), calorimetric DSC and preliminary X-ray measurements on the fifth member - 5.OAOB - of the alkoxyazoxybenzene homologous series are presented. It has been found that 5.OAOB exhibits two mesophases: a nematic (N) and an ''intermediate'' crystalline phase (Cr I) just below it. From comparison of the DR and QNS studies one can conclude that in the N phase the molecule as a whole performs rotational diffusion around the long axis (τ perpendicular DR ∼150 ps) and at the same time the two moieties perform faster independent reorientations around N - benzene rings bonds with τ QNS ∼5 ps. The Cr I phase is identified as a solid unaxial rotational phase in which fast molecular reorientations exist. It seems that the fast reorientations observed in the N phase to some extent survive to the Cr I phase. A model of molecular arrangements in the Cr I phase is proposed and it explains the reduction of the dielectric increment observed on passing from the N phase to this phase. (author)

A structural phase transition coupled to the Fe{sup 3+} spin-state crossover in anhydrous RbMn[Fe(CN){sub 6}

Energy Technology Data Exchange (ETDEWEB)

Rykov, A. I., E-mail: rykov3@yahoo.com; Wang, J., E-mail: wangjh@dicp.ac.cn; Zhang, T. [Chinese Academy of Sciences, Moessbauer Effect Data Center, Dalian Institute of Chemical Physics (China); Nomura, K. [University of Tokyo, Graduate School of Engineering (Japan)

2013-04-15

Linkage isomerism is the coexistence of iso-compositional molecules or solids differing by connectivity of the metal to a ligand. In a crystalline solid state, the rotation is possible for asymmetric ligands, e.g., for cyanide ligand. Here we report on our observation of a phase transition in anhydrous RbMn[Fe(CN){sub 6}] (nearly stoichiometric) and on the effect of linkage isomerism ensuing our interpretation of the results of Moessbauer study in which we observe the iron spin state crossover among two phases involved into this transition. The anhydrous RbMn[Fe(CN){sub 6}] can be prepared via prolonged thermal treatment (1 week at at 80 Degree-Sign C) of the as-synthesized hydrated RbMn[Fe(CN){sub 6}]{center_dot}H{sub 2}O. The latter compound famous for its charge-transfer phase transition is a precursor in our case. As the temperature is raising above 80 Degree-Sign C (remaining below 100 Degree-Sign C) we observe RbMn[Fe(CN){sub 6}] that inherited its F-43 m symmetry from RbMn[Fe(CN){sub 6}]{center_dot}H{sub 2}O transforming to a phase of the Fm-3 m symmetry. In the latter, more than half of Fe{sup 3 + } ions are in high-spin state. We suggest a plausible way to explain the spin-crossover that is to allow the linkage isomerism by rotation of the cyanide ligands.

Coherent spin transport through a 350 micron thick silicon wafer.

Science.gov (United States)

Huang, Biqin; Monsma, Douwe J; Appelbaum, Ian

2007-10-26

We use all-electrical methods to inject, transport, and detect spin-polarized electrons vertically through a 350-micron-thick undoped single-crystal silicon wafer. Spin precession measurements in a perpendicular magnetic field at different accelerating electric fields reveal high spin coherence with at least 13pi precession angles. The magnetic-field spacing of precession extrema are used to determine the injector-to-detector electron transit time. These transit time values are associated with output magnetocurrent changes (from in-plane spin-valve measurements), which are proportional to final spin polarization. Fitting the results to a simple exponential spin-decay model yields a conduction electron spin lifetime (T1) lower bound in silicon of over 500 ns at 60 K.

Field-induced phase transition in a metalorganic spin-dimer system-a potential model system to study Bose-Einstein condensation of magnons

International Nuclear Information System (INIS)

Tsui, Y.; Bruehl, A.; Removic-Langer, K.; Pashchenko, V.; Wolf, B.; Donath, G.; Pikul, A.; Kretz, T.; Lerner, H.-W.; Wagner, M.; Salguero, A.; Saha-Dasgupta, T.; Rahaman, B.; Valenti, R.; Lang, M.

2007-01-01

We report on the results obtained from studying electron spin resonance, magnetic susceptibility, specific heat and thermal expansion experiments on a metalorganic spin-dimer system, C 36 H 48 Cu 2 F 6 N 8 O 12 S 2 (TK91). According to the first principle Density Functional Theory calculations, the compound represents a 3D-coupled dimer system with intradimer coupling J 1 /k B ∼ 10K and interdimer couplings J 2 /k B ∼J 3 /k B ∼ 1K. The measurements have been performed on both pressed powder and single-crystal samples in external magnetic fields up to 12T and at low temperatures down to ∼ 0.2K. Susceptibility measurements reveal a spin-gap behavior consistent with the theoretical results. Furthermore, clear indications of a field-induced phase transition have been observed. A similar field-induced phase transition was also detected in an inorganic compound TlCuCl 3 and was interpreted as Bose-Einstein condensation (BEC) of magnons. The possibility of changing both the intradimer and interdimer couplings in TK91 by chemical substitutions makes the system a potentially good system to study BEC of magnons

Stress induced reorientation of vanadium hydride

International Nuclear Information System (INIS)

Beardsley, M.B.

1977-10-01

The critical stress for the reorientation of vanadium hydride was determined for the temperature range 180 0 to 280 0 K using flat tensile samples containing 50 to 500 ppM hydrogen by weight. The critical stress was observed to vary from a half to a third of the macroscopic yield stress of pure vanadium over the temperature range. The vanadium hydride could not be stress induced to precipitate above its stress-free precipitation temperature by uniaxial tensile stresses or triaxial tensile stresses induced by a notch

Stategic reorientation of industrial R&D towards commercial objectives.

NARCIS (Netherlands)

Brook, Jacques W.; de Bruijn, E.J.; McDonough III, Edward F.; Kaynak, E.; Harcar, T.D.

2007-01-01

In an effort to leverage R&D knowledge asset and to create more value from industrial R&D in today’s increasing liberalized and globalising business environments, some corporations adopt a strategic reorientation of their industrial R&D organisation towards commercial objectives. This study suggests

The reorientation of cell nucleus promotes the establishment of front-rear polarity in migrating fibroblasts.

Science.gov (United States)

Maninová, Miloslava; Klímová, Zuzana; Parsons, J Thomas; Weber, Michael J; Iwanicki, Marcin P; Vomastek, Tomáš

2013-06-12

The establishment of cell polarity is an essential step in the process of cell migration. This process requires precise spatiotemporal coordination of signaling pathways that in most cells create the typical asymmetrical profile of a polarized cell with nucleus located at the cell rear and the microtubule organizing center (MTOC) positioned between the nucleus and the leading edge. During cell polarization, nucleus rearward positioning promotes correct microtubule organizing center localization and thus the establishment of front-rear polarity and directional migration. We found that cell polarization and directional migration require also the reorientation of the nucleus. Nuclear reorientation is manifested as temporally restricted nuclear rotation that aligns the nuclear axis with the axis of cell migration. We also found that nuclear reorientation requires physical connection between the nucleus and cytoskeleton mediated by the LINC (linker of nucleoskeleton and cytoskeleton) complex. Nuclear reorientation is controlled by coordinated activity of lysophosphatidic acid (LPA)-mediated activation of GTPase Rho and the activation of integrin, FAK (focal adhesion kinase), Src, and p190RhoGAP signaling pathway. Integrin signaling is spatially induced at the leading edge as FAK and p190RhoGAP are predominantly activated or localized at this location. We suggest that integrin activation within lamellipodia defines cell front, and subsequent FAK, Src, and p190RhoGAP signaling represents the polarity signal that induces reorientation of the nucleus and thus promotes the establishment of front-rear polarity. Copyright © 2013 Elsevier Ltd. All rights reserved.

Spin-transfer torque generated by a topological insulator

KAUST Repository

Mellnik, A. R.

2014-07-23

Magnetic devices are a leading contender for the implementation of memory and logic technologies that are non-volatile, that can scale to high density and high speed, and that do not wear out. However, widespread application of magnetic memory and logic devices will require the development of efficient mechanisms for reorienting their magnetization using the least possible current and power. There has been considerable recent progress in this effort; in particular, it has been discovered that spin-orbit interactions in heavy-metal/ferromagnet bilayers can produce strong current-driven torques on the magnetic layer, via the spin Hall effect in the heavy metal or the Rashba-Edelstein effect in the ferromagnet. In the search for materials to provide even more efficient spin-orbit-induced torques, some proposals have suggested topological insulators, which possess a surface state in which the effects of spin-orbit coupling are maximal in the sense that an electron\\' s spin orientation is fixed relative to its propagation direction. Here we report experiments showing that charge current flowing in-plane in a thin film of the topological insulator bismuth selenide (Bi2Se3) at room temperature can indeed exert a strong spin-transfer torque on an adjacent ferromagnetic permalloy (Ni81Fe19) thin film, with a direction consistent with that expected from the topological surface state. We find that the strength of the torque per unit charge current density in Bi 2Se3 is greater than for any source of spin-transfer torque measured so far, even for non-ideal topological insulator films in which the surface states coexist with bulk conduction. Our data suggest that topological insulators could enable very efficient electrical manipulation of magnetic materials at room temperature, for memory and logic applications. © 2014 Macmillan Publishers Limited. All rights reserved.

Dynamic magnetic hysteresis behavior and dynamic phase transition in the spin-1 Blume-Capel model

Energy Technology Data Exchange (ETDEWEB)

Deviren, Bayram, E-mail: bayram.deviren@nevsehir.edu.tr [Department of Physics, Nevsehir University, 50300 Nevsehir (Turkey); Keskin, Mustafa [Department of Physics, Erciyes University, 38039 Kayseri (Turkey)

2012-03-15

The nature (time variation) of response magnetization m(wt) of the spin-1 Blume-Capel model in the presence of a periodically varying external magnetic field h(wt) is studied by employing the effective-field theory (EFT) with correlations as well as the Glauber-type stochastic dynamics. We determine the time variations of m(wt) and h(wt) for various temperatures, and investigate the dynamic magnetic hysteresis behavior. We also investigate the temperature dependence of the dynamic magnetization, hysteresis loop area and correlation near the transition point in order to characterize the nature (first- or second-order) of the dynamic transitions as well as obtain the dynamic phase transition temperatures. The hysteresis loops are obtained for different reduced temperatures and we find that the areas of the loops are decreasing with the increasing of the reduced temperatures. We also present the dynamic phase diagrams and compare the results of the EFT with the results of the dynamic mean-field approximation. The phase diagrams exhibit many dynamic critical points, such as tricritical ( Bullet ), zero-temperature critical (Z), triple (TP) and multicritical (A) points. According to values of Hamiltonian parameters, besides the paramagnetic (P), ferromagnetic (F) fundamental phases, one coexistence or mixed phase region, (F+P) and the reentrant behavior exist in the system. The results are in good agreement with some experimental and theoretical results. - Highlights: Black-Right-Pointing-Pointer Kinetic spin-1 Blume-Capel model is studied using the effective-field theory. Black-Right-Pointing-Pointer We investigated the dynamic magnetic hysteresis behavior. Black-Right-Pointing-Pointer Dynamic magnetization, hysteresis loop area and correlation are investigated. Black-Right-Pointing-Pointer System exhibits tricritical, zero-temperature, triple and multicritical points. Black-Right-Pointing-Pointer We present the dynamic phase diagrams and compare the results of the EFT

Spontaneous spin-polarization and phase transition in the relativistic approach

International Nuclear Information System (INIS)

Maruyama, Tomoyuki; Tatsumi, Toshitaka

2001-01-01

We study the spin-polarization mechanism in the highly dense nuclear matter with the relativistic mean-field approach. In the relativistic Hartree-Fock framework we find that there are two kinds of spin-spin interaction channels, which are the axial-vector and tensor exchange ones. If each interaction is strong and different sign, the system loses the spherical symmetry and holds the spin-polarization in the high-density region. When the axial-vector interaction is negative enough, the system holds ferromagnetism. (author)

Fluorescence quenching studies of potential-dependent DNA reorientation dynamics at glassy carbon electrode surfaces.

Science.gov (United States)

Li, Qin; Cui, Chenchen; Higgins, Daniel A; Li, Jun

2012-09-05

The potential-dependent reorientation dynamics of double-stranded DNA (ds-DNA) attached to planar glassy carbon electrode (GCE) surfaces were investigated. The orientation state of surface-bound ds-DNA was followed by monitoring the fluorescence from a 6-carboxyfluorescein (FAM6) fluorophore covalently linked to the distal end of the DNA. Positive potentials (i.e., +0.2 V vs open circuit potential, OCP) caused the ds-DNA to align parallel to the electrode surface, resulting in strong dipole-electrode quenching of FAM6 fluorescence. Switching of the GCE potential to negative values (i.e., -0.2 V vs OCP) caused the ds-DNA to reorient perpendicular to the electrode surface, with a concomitant increase in FAM6 fluorescence. In addition to the very fast (submilliseconds) dynamics of the initial reorientation process, slow (0.1-0.9 s) relaxation of FAM6 fluorescence to intermediate levels was also observed after potential switching. These dynamics have not been previously described in the literature. They are too slow to be explained by double layer charging, and chronoamperometry data showed no evidence of such effects. Both the amplitude and rate of the dynamics were found to depend upon buffer concentration, and ds-DNA length, demonstrating a dependence on the double layer field. The dynamics are concluded to arise from previously undetected complexities in the mechanism of potential-dependent ds-DNA reorientation. The possible origins of these dynamics are discussed. A better understanding of these dynamics will lead to improved models for potential-dependent ds-DNA reorientation at electrode surfaces and will facilitate the development of advanced electrochemical devices for detection of target DNAs.

Spin crossover and high spin filtering behavior in Co-Pyridine and Co-Pyrimidine molecules

Science.gov (United States)

Wen, Zhongqian; Zhou, Liping; Cheng, Jue-Fei; Li, Shu-Jin; You, Wen-Long; Wang, Xuefeng

2018-03-01

We present a theoretical study on a series of cobalt complexes, which are constructed with cobalt atoms and pyridine/pyrimidine rings, using density functional theory. We investigate the structural and electric transport properties of spin crossover (SCO) Co complex with two spin states, namely low-spin configuration [LS] and high-spin configuration [HS]. Energy analyses of the two spin states imply that the SCO Co-Pyridine2 and Co-Pyrimidine2 complexes may display a spin transition process accompanied by a geometric modification driven by external stimuli. A nearly perfect spin filtering effect is observed in the Co-Pyrimidine2 complex with [HS] state. In addition, we also discover the contact-dependent transmission properties of Co-Pyridine2. These findings indicate that SCO Co complexes are promising materials for molecular spintronic devices.

Photoinduced reorientation and polarization holography in a new photopolymer with 4-methoxy-N-benzylideneaniline side groups

Directory of Open Access Journals (Sweden)

Nobuhiro Kawatsuki

2013-08-01

Full Text Available The photoinduced reorientation and surface relief (SR formation behaviors of a novel photosensitive polymer, which was transparent in visible region, were investigated using linearly polarized-313-nm light and holographic exposure with a 325-nm He-Cd laser. The polymer was comprised of photosensitive 4-methoxy-N-benzylideneaniline side groups, and exhibited a sufficient photoinduced molecular reorientation with a birefringence of 0.11. Holographic exposure generated a SR structure, which had a periodical molecular reorientation that depended on the polarization of the interference beams. The generated SR height was ∼212 nm, and the inscription of a double holographic exposure yielded a two-dimensional SR structure.

Reorientation of single-wall carbon nanotubes in negative anisotropy liquid crystals by an electric field

Directory of Open Access Journals (Sweden)

Amanda García-García

2016-06-01

Full Text Available Single-wall carbon nanotubes (SWCNT are anisotropic nanoparticles that can cause modifications in the electrical and electro-optical properties of liquid crystals. The control of the SWCNT concentration, distribution and reorientation in such self-organized fluids allows for the possibility of tuning the liquid crystal properties. The alignment and reorientation of CNTs are studied in a system where the liquid crystal orientation effect has been isolated. Complementary studies including Raman spectroscopy, microscopic inspection and impedance studies were carried out. The results reveal an ordered reorientation of the CNTs induced by an electric field, which does not alter the orientation of the liquid crystal molecules. Moreover, impedance spectroscopy suggests a nonnegligible anchoring force between the CNTs and the liquid crystal molecules.

Pressure-induced spin and charge transport in La1.25Sr1.75Mn2O7 single crystal

International Nuclear Information System (INIS)

Mydeen, K.; Arumugam, S.; Prabhakaran, D.; Yu, R.C.; Jin, C.Q.

2009-01-01

We investigated the effect of uniaxial and hydrostatic pressure on resistivity and ac-magnetic susceptibility of two-dimensional layered manganite, La 1.25 Sr 1.75 Mn 2 O 7 (LSMO125) to investigate the lattice effect on magnetic and electronic properties. Asymmetric role of uniaxial pressure, || and -perpendicular to c-axis on the spin flop and charge transport has been revealed while comparing hydrostatic pressure. Uniaxial pressure along c-axis increases metal-insulator transition temperature (T MI ) and ferromagnetic ordering temperature (T C ), whereas it decreases the resistivity along ab-plane (ρ ab ). In contrast to pressure along c-axis, T MI and T C decrease, whereas the resistivity along c-axis (ρ c ) increases with pressure || to ab-plane. ρ c /ρ ab is quite large, increasing with pressure and shows a peak at around T MI . Uniaxial pressure behaviour is strongly related to the Mn-O-Mn linkage between MnO 2 layers and the spin reorientation from the apical axis to the basal plane and vice versa with pressure. Both ρ ab and ρ c decrease whereas T MI and T C increases under hydrostatic pressure. Influence of spin and charge on magnetic and electrical properties under hydrostatic pressure are explained by pressure-induced cant between the MnO 2 bilayers and variation in bond lengths. The different pressure driving rates of T MI while measuring ρ ab and ρ c confirms that there is a strong competition between the in and out plane components under hydrostatic pressure

Novel spin transition between S = 5/2 and S = 3/2 in highly saddled iron(III) porphyrin complexes at extremely low temperatures.

Science.gov (United States)

Ohgo, Yoshiki; Chiba, Yuya; Hashizume, Daisuke; Uekusa, Hidehiro; Ozeki, Tomoji; Nakamura, Mikio

2006-05-14

A novel spin transition between S = 5/2 and S = 3/2 has been observed for the first time in five-coordinate, highly saddled iron(III) porphyrinates by EPR and SQUID measurements at extremely low temperatures.

The Kubo-Greenwood spin-dependent electrical conductivity of 2D transition-metal dichalcogenides and group-IV materials: A Green's function study

Science.gov (United States)

Hoi, Bui Dinh; Yarmohammadi, Mohsen

2018-04-01

The spin-dependent electrical conductivity of counterparts of graphene, transition-metal dichalcogenides (TMDs) and group-IV nanosheets, have investigated by a magnetic exchange field (MEF)-induction to gain the electronic transport properties of charge carriers. We have implemented a k.p Hamiltonian model through the Kubo-Greenwood formalism in order to address the dynamical behavior of correlated Dirac fermions. Tuning the MEF enables one to control the effective mass of carriers in group-IV and TMDs, differently. We have found the Dirac-like points in a new quantum anomalous Hall (QAH) state at strong MEFs for both structures. For both cases, a broad peak in electrical conductivity originated from the scattering rate and entropy is observed. Spin degeneracy at some critical MEFs is another remarkable point. We have found that in the limit of zero or uniform MEFs with respect to the spin-orbit interaction, the large resulting electrical conductivity depends on the spin sub-bands in group-IV and MLDs. Featuring spin-dependent electronic transport properties, one can provide a new scenario for future possible applications.

Spin-Glass Transition and Giant Paramagnetism in Heavily Hole-Doped Bi2Sr2Co2Oy

Science.gov (United States)

Hsu, Hung Chang; Lee, Wei-Li; Lin, Jiunn-Yuan; Young, Ben-Li; Kung, Hsiang-Hsi; Huang, Jian; Chou, Fang Cheng

2014-02-01

Hole-doped single crystals of misfit-layered cobaltate Bi2-xPbxSr2-zCo2Oy (x = 0-0.61, y = 8.28-8.62, and z = 0.01-0.22) have been successfully grown using the optical floating-zone method. Heavier hole doping has been achieved through both Pb substitution in the Bi site and the more effective Sr vacancy formation. The Co4+ : Co3+ ratio can be raised significantly from its original ˜1 : 1 to 4.5 : 1, as confirmed by iodometric titration. A spin-glass transition temperature of Tg ˜ 70 K is confirmed by ac susceptibility measurement when the Co4+ : Co3+ ratio becomes higher than 2 : 1, presumably owing to the significantly increased probability of triangular geometrical frustration among antiferromagnetically coupled localized Co4+ spins.

Nuclear Spin Nanomagnet in an Optically Excited Quantum Dot

Science.gov (United States)

Korenev, V. L.

2007-12-01

Linearly polarized light tuned slightly below the optical transition of the negatively charged exciton (trion) in a single quantum dot causes the spontaneous nuclear spin polarization (self-polarization) at a level close to 100%. The effective magnetic field of spin-polarized nuclei shifts the optical transition energy close to resonance with photon energy. The resonantly enhanced Overhauser effect sustains the stability of the nuclear self-polarization even in the absence of spin polarization of the quantum dot electron. As a result the optically selected single quantum dot represents a tiny magnet with the ferromagnetic ordering of nuclear spins—the nuclear spin nanomagnet.

Microtubule array reorientation in response to hormones does not involve changes in microtubule nucleation modes at the periclinal cell surface

Science.gov (United States)

Atkinson, Samantha; Kirik, Angela; Kirik, Viktor

2014-01-01

Aligned microtubule arrays spatially organize cell division, trafficking, and determine the direction of cell expansion in plant cells. In response to changes in environmental and developmental signals, cells reorganize their microtubule arrays into new configurations. Here, we tested the role of microtubule nucleation during hormone-induced microtubule array reorientation. We have found that in the process of microtubule array reorientation the ratios between branching, parallel, and de-novo nucleations remained constant, suggesting that the microtubule reorientation mechanism does not involve changes in nucleation modes. In the ton2/fass mutant, which has reduced microtubule branching nucleation frequency and decreased nucleation activity of the γ-tubulin complexes, microtubule arrays were able to reorient. Presented data suggest that reorientation of microtubules into transverse arrays in response to hormones does not involve changes in microtubule nucleation at the periclinal cell surface PMID:25135522

Identification of high-spin states in 235U

International Nuclear Information System (INIS)

Lorenz, A.; Makarenko, V.E.; Chukreev, F.E.

1994-02-01

The results of a 235 U high spin states study are analysed. A new way to assign newly observed gamma ray transitions is proposed. Such assignments deals with low spin parts of the level scheme without introducing high spin level states. (author)

Spin polarized states in strongly asymmetric nuclear matter

International Nuclear Information System (INIS)

Isayev, A.A.; Yang, J.

2004-01-01

The possibility of appearance of spin polarized states in strongly asymmetric nuclear matter is analyzed within the framework of a Fermi liquid theory with the Skyrme effective interaction. The zero temperature dependence of the neutron and proton spin polarization parameters as functions of density is found for SLy4 and SLy5 effective forces. It is shown that at some critical density strongly asymmetric nuclear matter undergoes a phase transition to the state with the oppositely directed spins of neutrons and protons while the state with the same direction of spins does not appear. In comparison with neutron matter, even small admixture of protons strongly decreases the threshold density of spin instability. It is clarified that protons become totally polarized within a very narrow density domain while the density profile of the neutron spin polarization parameter is characterized by the appearance of long tails near the transition density

Direct observation of spin-quadrupolar excitations in Sr2CoGe2O7 by high-field electron spin resonance

Science.gov (United States)

Akaki, Mitsuru; Yoshizawa, Daichi; Okutani, Akira; Kida, Takanori; Romhányi, Judit; Penc, Karlo; Hagiwara, Masayuki

2017-12-01

Exotic spin-multipolar ordering in spin transition metal insulators has so far eluded unambiguous experimental observation. A less studied, but perhaps more feasible fingerprint of multipole character emerges in the excitation spectrum in the form of quadrupolar transitions. Such multipolar excitations are desirable as they can be manipulated with the use of light or electric field and can be captured by means of conventional experimental techniques. Here we study single crystals of multiferroic Sr2CoGe2O7 and observe a two-magnon spin excitation appearing above the saturation magnetic field in electron spin resonance (ESR) spectra. Our analysis of the selection rules reveals that this spin excitation mode does not couple to the magnetic component of the light, but it is excited by the electric field only, in full agreement with the theoretical calculations. Due to the nearly isotropic nature of Sr2CoGe2O7 , we identify this excitation as a purely spin-quadrupolar two-magnon mode.

Spin interferometry in anisotropic spin-orbit fields

Science.gov (United States)

Saarikoski, Henri; Reynoso, Andres A.; Baltanás, José Pablo; Frustaglia, Diego; Nitta, Junsaku

2018-03-01

Electron spins in a two-dimensional electron gas can be manipulated by spin-orbit (SO) fields originating from either Rashba or Dresselhaus interactions with independent isotropic characteristics. Together, though, they produce anisotropic SO fields with consequences on quantum transport through spin interference. Here we study the transport properties of modeled mesoscopic rings subject to Rashba and Dresselhaus [001] SO couplings in the presence of an additional in-plane Zeeman field acting as a probe. By means of one- and two-dimensional quantum transport simulations we show that this setting presents anisotropies in the quantum resistance as a function of the Zeeman field direction. Moreover, the anisotropic resistance can be tuned by the Rashba strength up to the point to invert its response to the Zeeman field. We also find that a topological transition in the field texture that is associated with a geometric phase switching is imprinted in the anisotropy pattern. We conclude that resistance anisotropy measurements can reveal signatures of SO textures and geometric phases in spin carriers.

Ordering phenomena in transition-metal-oxide heterostructures

International Nuclear Information System (INIS)

Frano Pereira, Alex Manuel

2014-01-01

This doctoral work presents a study of ordered ground states of transition metal oxide compounds and multilayers using resonant elastic soft x-ray scattering. The technique has developed over the last decades and become especially useful when sample sizes are limited like the case of nanometer-scale films and superlattices. By scattering with photon energies on resonance with the element's electronic transitions, it is an element-specific, sensitive tool providing a combination of spectroscopic and spatial information. The thesis is divided into two central topics. The first part focuses on the investigation of perovskite-type, rare-earth nickelate heterostructures. X-rays tuned to the Ni L 3 -edge were used to unveil unprecedented diffraction evidence of long range magnetic order in LaNiO 3 -RXO 3 (RXO 3 = LaAlO 3 , DyScO 3 ) superlattices. We report on the appearance of magnetic order in such systems with a propagation vector of Q SDW = ((1)/(4),(1)/(4),l) in pseudocubic notation, similar to bulk rare earth nickelates with R ≠ La. With LaNiO 3 being paramagnetic in its bulk form, the magnetic Bragg peak is only present in superlattices where the thickness of the LaNiO 3 layers approaches the 2-dimensional limit. Besides the thickness dependence, the magnetic order was probed on samples grown on varying strain-inducing substrates. Azimuthal scans around Q SDW were done to determine the orientation of the spin spiral under these different conditions. We will explain how the reorientation of the spins can be understood by the magneto-crystalline anisotropy which is determined by the relative occupation of the Ni d-orbitals via spin-orbit coupling. First steps towards control of the spin spiral's orientation will be outlined, and along with the high remanent conductivity found in the magnetic spiral state, an outlook for metallic antiferromagnetic spintronics will be discussed. The second part of this thesis will address the observation of charge density

Monte Carlo simulation and theory in Gaussian approximation of a phase transition in the nuclear spin system of a solid

Energy Technology Data Exchange (ETDEWEB)

Merkulov, I A; Papava, Y I; Ponomarenko, V V [Leningradskij Gosudarstvennyj Univ., Leningrad (Russian Federation); Vasiliev, S I [Carleton Univ., Ottawa, ON (Canada). Dept. of Physics

1988-02-01

A phase transition of the nuclear spin system of a solid with dipolar and indirect scalar interactions is considered. Monte Carlo simulations of the spin-system isothermic states and of the adiabatic demagnetization process have been made. The structures and energies of the ground states and the values of the critical temperatures, T[sub C], and minimal polarizations, [rho][sub C], at which adiabatic demagnetization leads to spontaneous spin ordering, calculated for the GaAs and CaF[sub 2] nuclear spin systems, are presented. The results of numerical simulations are compared with the experimental data for CaF[sub 2]. The Weiss-field model is extended to the case of adiabatic demagnetization. The fluctuations of the local field are taken into account in the Gaussian approximation. It is shown that the proposed approach allows one to obtain asymptotically correct results both for T >> T[sub C] and T << T[sub C]. The results of the calculations in the Gaussian approximation are compared with the numerical simulations. (10 refs., 9 figs., tab.).

Spin crossover and Mott—Hubbard transition under high pressure and high temperature in the low mantle of the Earth

Science.gov (United States)

Ovchinnikov, S. G.; Ovchinnikova, T. M.; Plotkin, V. V.; Dyad'kov, P. G.

2015-11-01

Effect of high pressure induced spin crossover on the magnetic, electronic and structural properties of the minerals forming the Earth's low mantle is discussed. The low temperature P, T phase diagram of ferropericlase has the quantum phase transition point Pc = 56 GPa at T = 0 confirmed recently by the synchrotron Mössbauer spectroscopy. The LDA+GTB calculated phase diagram describes the experimental data. Its extension to the high temperature resulted earlier in prediction of the metallic properties of the Earth's mantle at the depth 1400 km insulator transition and compare them with the experimental seismic and geomagnetic field data.

High-spin states and coexisting states in the Pt-Au transition region

International Nuclear Information System (INIS)

Riedinger, L.L.; Carpenter, M.P.; Courtney, L.H.; Janzen, V.P.; Schmitz, W.

1986-01-01

High-spin states in the N = 104 to 108 region have been studied by in-beam spectroscopy techniques in a number of Ir, Pt, and Au nuclei. These measurements have been performed at tandem Van de Graaff facilities at the Oak Ridge National Laboratory and at McMaster University. Through comparison of band crossings in a variety of odd-A and even-A nuclei, we are able to assign the first neutron and first proton alignment processes, which are nearly degenerate for 184 Pt. These measurements yield the trend of these crossing frequencies with N and Z in this region. Knowledge of this trend is important, since these crossing frequencies can give an estimate of how the shape parameters vary across this transitional region. 22 refs., 7 figs., 1 tab

Complex band structures of transition metal dichalcogenide monolayers with spin-orbit coupling effects

Science.gov (United States)

Szczęśniak, Dominik; Ennaoui, Ahmed; Ahzi, Saïd

2016-09-01

Recently, the transition metal dichalcogenides have attracted renewed attention due to the potential use of their low-dimensional forms in both nano- and opto-electronics. In such applications, the electronic and transport properties of monolayer transition metal dichalcogenides play a pivotal role. The present paper provides a new insight into these essential properties by studying the complex band structures of popular transition metal dichalcogenide monolayers (MX 2, where M  =  Mo, W; X  =  S, Se, Te) while including spin-orbit coupling effects. The conducted symmetry-based tight-binding calculations show that the analytical continuation from the real band structures to the complex momentum space leads to nonlinear generalized eigenvalue problems. Herein an efficient method for solving such a class of nonlinear problems is presented and yields a complete set of physically relevant eigenvalues. Solutions obtained by this method are characterized and classified into propagating and evanescent states, where the latter states manifest not only monotonic but also oscillatory decay character. It is observed that some of the oscillatory evanescent states create characteristic complex loops at the direct band gap of MX 2 monolayers, where electrons can directly tunnel between the band gap edges. To describe these tunneling currents, decay behavior of electronic states in the forbidden energy region is elucidated and their importance within the ballistic transport regime is briefly discussed.

Mechanisms of spin-flipping and metal-insulator transition in nano-Fe3O4

Science.gov (United States)

Dito Fauzi, Angga; Aziz Majidi, Muhammad; Rusydi, Andrivo

2017-04-01

Fe3O4 is a half-metallic ferrimagnet with {{T}\\text{C}}˜ 860 K exhibiting metal-insulator transition (MIT) at  ˜120 K. In bulk form, the saturation magnetization is 0.6 Tesla (˜471 emu cm-3). A recent experimental study has shown that the saturation magnetization of nano-Fe3O4 thin films can achieve up to  ˜760 emu cm-3, attributed to spin-flipping of Fe ions at tetrahedral sites assisted by oxygen vacancies (V O). Such a system has shown to have higher MIT temperature (˜150 K). The spin-flipping is a new phenomenon in Fe3O4, while the MIT is a long-standing one. Here, we propose a model and calculations to investigate the mechanisms of both phenomena. Our results show that, for the system without V O, the ferrimagnetic configuration is energetically favorable. Remakably, upon inclusion of V O, the ground-state configuration switches into ferromagnetic. As for the MIT, by proposing temperature dependences of some hopping integrals in the model, we demonstrate that the system without and with V O undergo the MIT in slightly different ways, leading to higher MIT temperature for the system with V O, in agreement with the experimental data. Our results also show that the MIT in both systems occur concomitantly with the redistribution of electrons among the three Fe ions in each Fe3O4 formula unit. As such temperature dependences of hopping integrals may arise due to dynamic Jahn-Teller effects, our phenomenological theory may provide a way to reconcile existing theories relating the MIT to the structural transition and the charge ordering.

Tuning the presence of dynamical phase transitions in a generalized XY spin chain.

Science.gov (United States)

Divakaran, Uma; Sharma, Shraddha; Dutta, Amit

2016-05-01

We study an integrable spin chain with three spin interactions and the staggered field (λ) while the latter is quenched either slowly [in a linear fashion in time (t) as t/τ, where t goes from a large negative value to a large positive value and τ is the inverse rate of quenching] or suddenly. In the process, the system crosses quantum critical points and gapless phases. We address the question whether there exist nonanalyticities [known as dynamical phase transitions (DPTs)] in the subsequent real-time evolution of the state (reached following the quench) governed by the final time-independent Hamiltonian. In the case of sufficiently slow quenching (when τ exceeds a critical value τ_{1}), we show that DPTs, of the form similar to those occurring for quenching across an isolated critical point, can occur even when the system is slowly driven across more than one critical point and gapless phases. More interestingly, in the anisotropic situation we show that DPTs can completely disappear for some values of the anisotropy term (γ) and τ, thereby establishing the existence of boundaries in the (γ-τ) plane between the DPT and no-DPT regions in both isotropic and anisotropic cases. Our study therefore leads to a unique situation when DPTs may not occur even when an integrable model is slowly ramped across a QCP. On the other hand, considering sudden quenches from an initial value λ_{i} to a final value λ_{f}, we show that the condition for the presence of DPTs is governed by relations involving λ_{i},λ_{f}, and γ, and the spin chain must be swept across λ=0 for DPTs to occur.

Magnetic phase transitions and large magnetic entropy change with a wide temperature span in HoZn

Energy Technology Data Exchange (ETDEWEB)

Li, Lingwei, E-mail: wei0396@hotmail.com [Key Laboratory of Electromagnetic Processing of Materials (Ministry of Education), Northeastern University, Shenyang 110819 (China); Institut für Anorganische und Analytische Chemie, Universität Münster, Corrensstrasse 30, D-48149 Münster (Germany); Yuan, Ye [Helmholtz-Zentrum Dresden-Rossendorf (HZDR), Institute of Ion Beam Physics and Materials Research, P.O. Box 510119, 01314 Dresden (Germany); Zhang, Yikun [Key Laboratory of Electromagnetic Processing of Materials (Ministry of Education), Northeastern University, Shenyang 110819 (China); Pöttgen, Rainer [Institut für Anorganische und Analytische Chemie, Universität Münster, Corrensstrasse 30, D-48149 Münster (Germany); Zhou, Shengqiang [Helmholtz-Zentrum Dresden-Rossendorf (HZDR), Institute of Ion Beam Physics and Materials Research, P.O. Box 510119, 01314 Dresden (Germany)

2015-09-15

Highlights: • Magnetic phase transitions and magnetocaloric effect in HoZn were studied. • The critical properties of HoZn were systematically investigated. • The obtained critical exponents are satisfied with scaling theory. • A large reversible magnetocaloric effect in HoZn was observed. • HoZn could be a promising candidate for magnetic refrigeration. - Abstract: CsCl-type HoZn undergoes two successive magnetic phase transitions: (i) paramagnetic to ferromagnetic (FM) at T{sub C} ∼ 72 K and (ii) a spin reorientation (SR) at T{sub SR} ∼ 26 K. Magnetization and modified Arrott plots indicate that HoZn undergoes a second-order magnetic phase transition around T{sub C}. The obtained critical exponents have some small deviations from the mean-field theory, indicating a short range or a local magnetic interaction which is properly related to the coexistence of FM and SR transitions at low temperature. Two successive magnetic transitions in HoZn induce one broad pronounced peak together with a shoulder in the temperature dependence of the magnetic entropy change −ΔS{sub M}(T) curves, resulting in a wide temperature range with a large relative cooling power (RCP). For a field change of 0–7 T, the maximum value of −ΔS{sub M} is 15.2 J/kg K around T{sub C} with a large RCP value of 1124 J/kg. The large reversible magnetocaloric effect (MCE) and RC indicate that HoZn is a good candidate for active magnetic refrigeration.

Quantum statistical metastability for a finite spin

Science.gov (United States)

Garanin, D. A.; Chudnovsky, E. M.

2001-01-01

We study quantum-classical escape-rate transitions for uniaxial and biaxial models with finite spins S=10 (such as Mn12Ac and Fe8) and S=100 by a direct numerical approach. At second-order transitions the level making a dominant contribution into thermally assisted tunneling changes gradually with temperature whereas at first-order transitions a group of levels is skipped. For finite spins, the quasiclassical boundaries between first- and second-order transitions are shifted, favoring a second-order transition: For Fe8 in zero field the transition should be first order according to a theory with S-->∞, but we show that there are no skipped levels at the transition. Applying a field along the hard axis in Fe8 makes transition the strongest first order. For the same model with S=100 we confirmed the existence of a region where a second-order transition is followed by a first-order transition [X. Martínes Hidalgo and E. M. Chudnovsky, J. Phys.: Condensed Matter 12, 4243 (2000)].

Stable panoramic views facilitate snap-shot like memories for spatial reorientation in homing pigeons.

Directory of Open Access Journals (Sweden)

Tommaso Pecchia

Full Text Available Following spatial disorientation, animals can reorient themselves by relying on geometric cues (metric and sense specified both by the macroscopic surface layout of an enclosed space and prominent visual landmarks in arrays. Whether spatial reorientation in arrays of landmarks is based on explicit representation of the geometric cues is a matter of debate. Here we trained homing pigeons (Columba livia to locate a food-reward in a rectangular array of four identical or differently coloured pipes provided with four openings, only one of which allowed the birds to have access to the reward. Pigeons were trained either with a stable or a variable position of the opening on pipes, so that they could view the array either from the same or a variable perspective. Explicit mapping of configural geometry would predict successful reorientation irrespective of access condition. In contrast, we found that a stable view of the array facilitated spatial learning in homing pigeons, likely through the formation of snapshot-like memories.

Spontaneous reorientation is guided by perceived surface distance, not by image matching or comparison.

Directory of Open Access Journals (Sweden)

Sang Ah Lee

Full Text Available Humans and animals recover their sense of position and orientation using properties of the surface layout, but the processes underlying this ability are disputed. Although behavioral and neurophysiological experiments on animals long have suggested that reorientation depends on representations of surface distance, recent experiments on young children join experimental studies and computational models of animal navigation to suggest that reorientation depends either on processing of any continuous perceptual variables or on matching of 2D, depthless images of the landscape. We tested the surface distance hypothesis against these alternatives through studies of children, using environments whose 3D shape and 2D image properties were arranged to enhance or cancel impressions of depth. In the absence of training, children reoriented by subtle differences in perceived surface distance under conditions that challenge current models of 2D-image matching or comparison processes. We provide evidence that children's spontaneous navigation depends on representations of 3D layout geometry.

Neutron diffraction study of single crystalline ErCo10Mo2

International Nuclear Information System (INIS)

Janssen, Y.; De Boer, F.R.; Brueck, E.; Tegus, O.; Ma, L.; Buschow, K.H.J.; Reehuis, M.

1999-01-01

Complete text of publication follows. The ferrimagnetic intermetallic compound ErCo 10 Mo 2 (Tc = 600 K) crystallizes in the tetragonal ThMn 12 -type structure (space group 14/mmm). The Co and Mo atoms may share three crystallographic sites (8f, 8i and 8j). Earlier neutron powder diffraction experiments show that Mo has a strong preference for the 8i-site and that the magnetic ordering at low temperature is planar. Furthermore ErCo 10 Mo 2 has been reported to show one [2] or more [3] spin-reorientation transitions from planar to axial magnetic ordering. Recently we succeeded in growing a single-crystalline sample of ErCo 10 Mo 2 . Magnetic measurements in 1T show one spin-reorientation transition at about 135 K. Neutron diffraction experiments were performed to investigate a possible link between the magnetic properties and the site occupation by Mo. Our results show that our sample has the Mo atoms exclusively occupying half the 8i-sites. There is no evidence for a crystallographic superstructure. Furthermore, below 150 K some reflections strongly increase due to the growing Er magnetic moment. (author)

Manipulating magnetic anisotropy of the ultrathin Co{sub 2}FeAl full-Heusler alloy film via growth orientation of the Pt buffer layer

Energy Technology Data Exchange (ETDEWEB)

Wen, F.S., E-mail: wenfsh03@126.com [State Key Lab of Metastable Materials Science and Technology, Yanshan University, Qinhuangdao 066004 (China); Xiang, J.Y.; Hao, C.X.; Zhang, F.; Lv, Y.F. [State Key Lab of Metastable Materials Science and Technology, Yanshan University, Qinhuangdao 066004 (China); Wang, W.H. [Institute of Physics, Chinese Academy of Science, Beijing 100080 (China); Hu, W.T.; Liu, Z.Y. [State Key Lab of Metastable Materials Science and Technology, Yanshan University, Qinhuangdao 066004 (China)

2013-12-15

The ultrathin films of Co{sub 2}FeAl (CFA) full-Heusler alloy were prepared between two Pt layers on MgO single crystals by magnetron sputtering. By controlling the substrate temperature, different growth orientations of the Pt underlayers were realized, and their effects were investigated on the magnetic anisotropy of the ultrathin CFA film. It was revealed that different Pt orientations lead to distinctly different magnetic anisotropy for the sandwiched ultrathin CFA films. The Pt (111) orientation favors the perpendicular anisotropy, while the appearance of partial Pt (001) orientation leads to the quick decrease of perpendicular anisotropy and the complete Pt (001) orientation gives rise to the in-plane anisotropy. With the Pt (111) orientation, the temperature and thickness-induced spin reorientation transitions were investigated in the sandwiched ultrathin CFA films. - Highlights: • Different Pt orientations lead to different magnetic anisotropy for sandwiched ultrathin CFA films. • The Pt (111) orientation favors the perpendicular anisotropy for CFA layer. • Temperature and thickness-induced spin reorientation transitions were investigated in sandwiched ultrathin CFA films. • 0.8 nm CFA film is good candidate as electrode in magnetic tunnel junctions.

Manipulating magnetic anisotropy of the ultrathin Co2FeAl full-Heusler alloy film via growth orientation of the Pt buffer layer

International Nuclear Information System (INIS)

Wen, F.S.; Xiang, J.Y.; Hao, C.X.; Zhang, F.; Lv, Y.F.; Wang, W.H.; Hu, W.T.; Liu, Z.Y.

2013-01-01

The ultrathin films of Co 2 FeAl (CFA) full-Heusler alloy were prepared between two Pt layers on MgO single crystals by magnetron sputtering. By controlling the substrate temperature, different growth orientations of the Pt underlayers were realized, and their effects were investigated on the magnetic anisotropy of the ultrathin CFA film. It was revealed that different Pt orientations lead to distinctly different magnetic anisotropy for the sandwiched ultrathin CFA films. The Pt (111) orientation favors the perpendicular anisotropy, while the appearance of partial Pt (001) orientation leads to the quick decrease of perpendicular anisotropy and the complete Pt (001) orientation gives rise to the in-plane anisotropy. With the Pt (111) orientation, the temperature and thickness-induced spin reorientation transitions were investigated in the sandwiched ultrathin CFA films. - Highlights: • Different Pt orientations lead to different magnetic anisotropy for sandwiched ultrathin CFA films. • The Pt (111) orientation favors the perpendicular anisotropy for CFA layer. • Temperature and thickness-induced spin reorientation transitions were investigated in sandwiched ultrathin CFA films. • 0.8 nm CFA film is good candidate as electrode in magnetic tunnel junctions

Magnetic ordering of CoCl2-GIC, a spin ceramic: hierarchical successive transitions and the intermediate glassy phase

International Nuclear Information System (INIS)

Suzuki, Masatsugu; Suzuki, Itsuko S; Matsuura, Motohiro

2007-01-01

Stage-2 CoCl 2 -graphite intercalation compound (GIC) is a spin ceramic which shows hierarchical successive transitions at T cu (= 8.9 K) and T cl (= 7.0 K) from the paramagnetic phase into an intra-cluster (two-dimensional ferromagnetic) order with inter-cluster disorder and then to an inter-cluster (three-dimensional antiferromagnetic like) order over the whole system. The nature of the inter-cluster disorder was suggested to be of spin glass by nonlinear magnetic response analyses around T cu and by studies on dynamical aspects of ordering between T cu and T cl . Here, we present a further extensive examination of a series of time dependence of zero-field cooled magnetization M ZFC after the ageing protocol below T cu . The time dependence of the relaxation rates S ZFC (t) = (1/H) dM ZFC (t)/dlnt dramatically changes from the curves of simple spin glass ageing effect below T cl to those of two peaks above T cl . The characteristic relaxation behaviour apparently indicates that there coexist two different kinds of glassy correlated region below T cu

Hysteresis, nucleation and growth phenomena in spin-crossover solids

Science.gov (United States)

Ridier, Karl; Molnár, Gábor; Salmon, Lionel; Nicolazzi, William; Bousseksou, Azzedine

2017-12-01

The observation and the study of first-order phase transitions in cooperative spin-crossover (SCO) solids exhibiting hysteresis behaviours are of particular interest and currently constitute a burgeoning area in the field of bistable molecular materials. The understanding and the control of the transition mechanisms (nucleation and growth processes) and their dynamics within the hysteresis region appear to be a general and appealing problem from a fundamental point of view and for technological applications as well. This review reports on the recent progresses and most important findings made on the spatiotemporal dynamics of the spin transition in SCO solids, particularly through the universal nucleation and growth process. Both thermally induced and light-induced spin transitions are discussed. We open up this review to the central question of the evolution of the transition mechanisms and dynamics in SCO nano-objects, which constitute promising systems to reach ultra-fast switching, and the experimental issues inherent to such studies at the micro- and nanometric scale.

Deformed Fredkin spin chain with extensive entanglement

Science.gov (United States)

Salberger, Olof; Udagawa, Takuma; Zhang, Zhao; Katsura, Hosho; Klich, Israel; Korepin, Vladimir

2017-06-01

We introduce a new spin chain which is a deformation of the Fredkin spin chain and has a phase transition between bounded and extensive entanglement entropy scaling. In this chain, spins have a local interaction of three nearest neighbors. The Hamiltonian is frustration-free and its ground state can be described analytically as a weighted superposition of Dyck paths that depends on a deformation parameter t. In the purely spin 1/2 case, whenever t\

Structural transition in Mo{sub 3}Sb{sub 7} probed by muon spin relaxation

Energy Technology Data Exchange (ETDEWEB)

Tabata, Y. [Department of Materials Science and Engineering, Kyoto University, Kyoto 606-8501 (Japan); Koyama, T.; Kohara, T. [Graduate School of Material Science, University of Hyogo, Kamigori, Ako-gun, Hyogo 678-1297 (Japan); Watanabe, I. [Advanced Meson Science Laboratory, RIKEN Nishina Center, Wako, Saitama 351-0198 (Japan); Nakamura, H., E-mail: h.nakamura@ht8.ecs.kyoto-u.ac.j [Department of Materials Science and Engineering, Kyoto University, Kyoto 606-8501 (Japan)

2009-04-15

Longitudinal-field muSR measurements have been made for Mo{sub 3}Sb{sub 7} focusing on the nature of the structural transition recently found at T{sub S}approx =50K. Taking account of a critical behavior of the relaxation rate lambda at approxT{sub S}, together with the motional narrowing of the nuclear dipolar field revealed in a zero-field experiment, and the tetragonal lattice symmetry lowering below T{sub S}, we propose long-range order of spin-singlet dimers, i.e., the formation of the valence bond crystal below T{sub S}. As a possible origin, the frustration in the interdimer antiferromagnetic interaction is suggested.

Electron spin-lattice relaxation in fractals

International Nuclear Information System (INIS)

Shrivastava, K.N.

1986-08-01

We have developed the theory of the spin-fracton interaction for paramagnetic ions in fractal structures. The interaction is exponentially damped by the self-similarity length of the fractal and by the range dimensionality d Φ . The relaxation time of the spin due to the absorption and emission of the fracton has been calculated for a general dimensionality called the Raman dimensionality d R , which for the fractons differs from the Hausdorff (fractal) dimensionality, D, as well as from the Euclidean dimensionality, d. The exponent of the energy level separation in the relaxation rate varies with d R d Φ /D. We have calculated the spin relaxation rate due to a new type of Raman process in which one fracton is absorbed to affect a spin transition from one electronic level to another and later another fracton is emitted along with a spin transition such that the difference in the energies of the two fractons is equal to the electronic energy level separation. The temperature and the dimensionality dependence of such a process has been found in several approximations. In one of the approximations where the van Vleck relaxation rate for a spin in a crystal is known to vary with temperature as T 9 , our calculated variation for fractals turns out to be T 6.6 , whereas the experimental value for Fe 3+ in frozen solutions of myoglobin azide is T 6.3 . Since we used d R =4/3 and the fracton range dimensionality d Φ =D/1.8, we expect to measure the dimensionalities of the problem by measuring the temperature dependence of the relaxation times. We have also calculated the shift of the paramagnetic resonance transition for a spin in a fractal for general dimensionalities. (author)

Spin critical opalescence in zero-temperature Bose-Einstein condensates

Science.gov (United States)

Santamore, D. H.; Timmermans, E.

2012-02-01

Cold-atom developments suggest the prospect of measuring scaling properties and long-range fluctuations of continuous phase transitions at zero temperature. We discuss the conditions for characterizing the phase separation of Bose-Einstein condensates of boson atoms in two distinct hyperfine spin states. The mean-field description breaks down as the system approaches the transition from the miscible side. An effective spin description clarifies the ferromagnetic nature of the transition. We show that a difference in the scattering lengths for the bosons in the same spin state leads to an effective internal magnetic field. The point at which the internal magnetic field vanishes (i.e., equal values of the like-boson scattering lengths) is a special point. We show that the long-range density fluctuations are suppressed near that point, while the effective spin exhibits the long-range fluctuations that characterize critical points. The zero-temperature system exhibits critical opalescence with respect to long-wavelength waves of impurity atoms that interact with the bosons in a spin-dependent manner.

The spin-Peierls chain revisited

International Nuclear Information System (INIS)

Hager, Georg; Weisse, Alexander; Wellein, Gerhard; Jeckelmann, Eric; Fehske, Holger

2007-01-01

We extend previous analytical studies of the ground-state phase diagram of a one-dimensional Heisenberg spin chain coupled to optical phonons, which for increasing spin-lattice coupling undergoes a quantum phase transition from a gapless to a gaped phase with finite lattice dimerisation. We check the analytical results against established four-block and new two-block density matrix renormalisation group (DMRG) calculations. Different finite-size scaling behaviour of the spin excitation gaps is found in the adiabatic and anti-adiabatic regimes

Mean-field theory of photoinduced molecular reorientation in azobenzene liquid crystalline side-chain polymers

DEFF Research Database (Denmark)

Pedersen, T.G.; Johansen, P.M.

1997-01-01

. The theory provides an explanation for the high long-term stability of the photoinduced anisotropy as well as a theoretical prediction of the temporal behavior of photoinduced birefringence. The theoretical results agree favorably with measurements in the entire range of writing intensities used......A novel mean-field theory of photoinduced reorientation and optical anisotropy in liquid crystalline side-chain polymers is presented and compared with experiments, The reorientation mechanism is based on photoinduced trans cis isomerization and a multidomain model of the material is introduced...

Universal spin dynamics in quantum wires

Energy Technology Data Exchange (ETDEWEB)

Fajardo, E. A.; Zülicke, U.; Winkler, R.

2017-10-01

We discuss the universal spin dynamics in quasi-one-dimensional systems including the real spin in narrow-gap semiconductors like InAs and InSb, the valley pseudospin in staggered single-layer graphene, and the combination of real spin and valley pseudospin characterizing single-layer transition metal dichalcogenides (TMDCs) such as MoS2, WS2, MoS2, and WSe2. All these systems can be described by the same Dirac-like Hamiltonian. Spin-dependent observable effects in one of these systems thus have counterparts in each of the other systems. Effects discussed in more detail include equilibrium spin currents, current-induced spin polarization (Edelstein effect), and spin currents generated via adiabatic spin pumping. Our work also suggests that a long-debated spin-dependent correction to the position operator in single-band models should be absent.

Quantum group spin nets: Refinement limit and relation to spin foams

Science.gov (United States)

Dittrich, Bianca; Martin-Benito, Mercedes; Steinhaus, Sebastian

2014-07-01

So far spin foam models are hardly understood beyond a few of their basic building blocks. To make progress on this question, we define analogue spin foam models, so-called "spin nets," for quantum groups SU(2)k and examine their effective continuum dynamics via tensor network renormalization. In the refinement limit of this coarse-graining procedure, we find a vast nontrivial fixed-point structure beyond the degenerate and the BF phase. In comparison to previous work, we use fixed-point intertwiners, inspired by Reisenberger's construction principle [M. P. Reisenberger, J. Math. Phys. (N.Y.) 40, 2046 (1999)] and the recent work [B. Dittrich and W. Kaminski, arXiv:1311.1798], as the initial parametrization. In this new parametrization fine-tuning is not required in order to flow to these new fixed points. Encouragingly, each fixed point has an associated extended phase, which allows for the study of phase transitions in the future. Finally we also present an interpretation of spin nets in terms of melonic spin foams. The coarse-graining flow of spin nets can thus be interpreted as describing the effective coupling between two spin foam vertices or space time atoms.

Spin waves and the order-disorder transition in chromium

DEFF Research Database (Denmark)

Als-Nielsen, Jens Aage; Dietrich, O.W.

1969-01-01

The inelastic magnetic scattering of neutrons has been studied in Cr and Cr0.95-Mn0.05 both below and above the Neel temperature. The temperature dependence of the spin-wave velocity in the alloy has been measured below TN. The scattering above TN may also be interpreted in terms of spin-wavelike...

Molecular reorientations in a substance with liquid-crystalline and plastic-crystalline phases

International Nuclear Information System (INIS)

Nguyen, Xuan Phuc.

1986-05-01

Results of dielectric relaxation (DR), quasielastic neutron scattering (QNS), far infrared absorption (FIR), proton magnetic resonance (PMR), differential scanning calorimetry (DSC) and preliminary X-ray diffraction measurements on the di-n-pentyloxyazoxybenzene (5.OAOB) are presented. The measurements carried out by all these methods showed that 5.OAOB exhibits a nontypical for liquid-crystalline materials phase diagram. It has two mesophases: a nematic (N) and an ''intermediate'' crystalline phase just below it. A complex interpretation of results obtained is given. All suggestions concerning the character of reorientational motions of the molecule as a whole as well as of its segments in mesomorphic phases are analyzed. From comparison of the DR and QNS studies one can conclude that in the N phase the molecule as a whole performs rotational diffusion around the long axis (τ DR ∼ 100 ps) and at the same time the two moieties perform faster independent reorientations around N - benzene rings bonds withτ QNS ∼ 5 ps. On the basis of various experimental data it is shown that the CrI phase is a plastic-crystalline phase for which the molecule and its segments perform fast stochastic unaxial reorientations. This is the first case where the existence of such a phase in liquid-crystalline materials has been experimentally confirmed. (author)

Experimental realization of a silicon spin field-effect transistor

OpenAIRE

Huang, Biqin; Monsma, Douwe J.; Appelbaum, Ian

2007-01-01

A longitudinal electric field is used to control the transit time (through an undoped silicon vertical channel) of spin-polarized electrons precessing in a perpendicular magnetic field. Since an applied voltage determines the final spin direction at the spin detector and hence the output collector current, this comprises a spin field-effect transistor. An improved hot-electron spin injector providing ~115% magnetocurrent, corresponding to at least ~38% electron current spin polarization after...

Possible evidence for spin-transfer torque induced by spin-triplet supercurrent

KAUST Repository

Li, Lailai

2017-10-04

Cooper pairs in superconductors are normally spin singlet. Nevertheless, recent studies suggest that spin-triplet Cooper pairs can be created at carefully engineered superconductor-ferromagnet interfaces. If Cooper pairs are spin-polarized they would transport not only charge but also a net spin component, but without dissipation, and therefore minimize the heating effects associated with spintronic devices. Although it is now established that triplet supercurrents exist, their most interesting property - spin - is only inferred indirectly from transport measurements. In conventional spintronics, it is well known that spin currents generate spin-transfer torques that alter magnetization dynamics and switch magnetic moments. The observation of similar effects due to spin-triplet supercurrents would not only confirm the net spin of triplet pairs but also pave the way for applications of superconducting spintronics. Here, we present a possible evidence for spin-transfer torques induced by triplet supercurrents in superconductor/ferromagnet/superconductor (S/F/S) Josephson junctions. Below the superconducting transition temperature T_c, the ferromagnetic resonance (FMR) field at X-band (~ 9.0 GHz) shifts rapidly to a lower field with decreasing temperature due to the spin-transfer torques induced by triplet supercurrents. In contrast, this phenomenon is absent in ferromagnet/superconductor (F/S) bilayers and superconductor/insulator/ferromagnet/superconductor (S/I/F/S) multilayers where no supercurrents pass through the ferromagnetic layer. These experimental observations are discussed with theoretical predictions for ferromagnetic Josephson junctions with precessing magnetization.

Transition currents in diagonal spin basis

International Nuclear Information System (INIS)

Rogalev, R.N.

1996-01-01

Scalar and pseudoscalar densities, vector, pseudovector and tensor currents are expressed in terms of momentum and spin vectors of the corresponding particles in an explicitly covariant way. The obtained expressions are free of singularities and make it possible to draw a number of identities, which relate axial-vector, vector and tensor currents to each other. 8 refs

Markov chain analysis of single spin flip Ising simulations

International Nuclear Information System (INIS)

Hennecke, M.

1997-01-01

The Markov processes defined by random and loop-based schemes for single spin flip attempts in Monte Carlo simulations of the 2D Ising model are investigated, by explicitly constructing their transition matrices. Their analysis reveals that loops over all lattice sites using a Metropolis-type single spin flip probability often do not define ergodic Markov chains, and have distorted dynamical properties even if they are ergodic. The transition matrices also enable a comparison of the dynamics of random versus loop spin selection and Glauber versus Metropolis probabilities

Reorientational motion of a cross-link junction in a poly(dimethylsiloxane) network measured by time-resolved fluorescence depolarization

International Nuclear Information System (INIS)

Stein, A.D.; Hoffman, D.A.; Frank, C.W.; Fayer, M.D.

1992-01-01

The reorientational dynamics of a cross-link junction in poly(dimethylsiloxane) networks, measured by the fluorescence anisotropy decay of a chromophore tagged to the cross-link, have been investigated over a range of temperatures from T g +75 to T g +150. The probe chromophore, 1-dimethylamino-5-sulfonylnaphthalene amide (dansyl amide), is pendant to a trifunctional silane that acts as a cross-linking molecule. In cyclohexanol, the fluorescence anisotropy decay is in agreement with Debye--Stokes--Einstein hydrodynamic theory (rotational diffusion) demonstrating that the cross-linker can be used as a probe of orientational relaxation. The fluorescence anisotropy decays at a rapid rate in an end-linked poly(dimethyl siloxane) network reflecting fast reorientational motion of the cross-link junction. This reorientation appears diffusive and has a temperature dependence in accord with the Williams--Landel--Ferry equation. A model is proposed that suggests that reorientation and translational motion of the cross-link occur simultaneously and are both coupled to fluctuations of the polymer chain ends

Study of the magnetic phase transitions and magnetocaloric effect in Dy{sub 2}Cu{sub 2}In compound

Energy Technology Data Exchange (ETDEWEB)

Zhang, Yikun, E-mail: ykzhang10@hotmail.com [State Key Laboratory of Advanced Special Steels, Shanghai University, Shanghai, 200072 (China); Shanghai Key Laboratory of Advanced Ferrometallurgy, Shanghai University, Shanghai, 200072 (China); School of Materials Science and Engineering, Shanghai University, 200072 (China); Institute of Materials Physics, University of Münster, Wilhelm-Klemm-Straße 10, D-48149, Münster (Germany); Xu, Xiao; Yang, Yang; Hou, Long; Ren, Zhongming [State Key Laboratory of Advanced Special Steels, Shanghai University, Shanghai, 200072 (China); Shanghai Key Laboratory of Advanced Ferrometallurgy, Shanghai University, Shanghai, 200072 (China); School of Materials Science and Engineering, Shanghai University, 200072 (China); Li, Xi, E-mail: lx_net@sina.com [State Key Laboratory of Advanced Special Steels, Shanghai University, Shanghai, 200072 (China); Shanghai Key Laboratory of Advanced Ferrometallurgy, Shanghai University, Shanghai, 200072 (China); School of Materials Science and Engineering, Shanghai University, 200072 (China); Wilde, Gerhard [Institute of Materials Physics, University of Münster, Wilhelm-Klemm-Straße 10, D-48149, Münster (Germany)

2016-05-15

The magnetic properties and magnetocaloric effect (MCE) in Dy{sub 2}Cu{sub 2}In compound have been investigated. Dy{sub 2}Cu{sub 2}In undergoes two magnetic phase transitions, a paramagnetic to ferromagnetic (FM) at T{sub C} ∼ 49.5 K followed by a spin reorientation (SR) at T{sub SR} ∼ 19.5 K. For a magnetic field change of 0–7 T, the maximum values of the magnetic entropy change (−ΔS{sub M}{sup max}) are estimated to be 16.5 around T{sub C} and 6.7 J/kg K around T{sub SR} with a large relative cooling power (RCP) value of 617 J/kg. The modified Arrott plots and universal curves of the rescaled ΔS{sub M} confirmed that the magnetic phase transitions in Dy{sub 2}Cu{sub 2}In compound belongs the second order phase transitions. The present results may provide some clues to search for new magnetocaloric materials belonging to RE{sub 2}T{sub 2}X system. - Highlights: • Magnetic properties and magnetocaloric effect in Dy{sub 2}Cu{sub 2}In was studied. • The Dy{sub 2}Cu{sub 2}In undergoes 2 s order magnetic phase transitions. • A large reversible MCE was observed in Dy{sub 2}Cu{sub 2}In. • The origin of MCE and its potential application in Dy{sub 2}Cu{sub 2}In were discussed.

New type of ordering process with volume change of molecules in the spin-crossover transition, and its new aspects of dynamical processes

Science.gov (United States)

Miyashita, Seiji; Nishino, Masamichi; Konishi, Yusuke; Tokoro, Hiroko; Boukheddaden, Kamel; Varret, François; Rikvold, Per Arne

2009-02-01

Bistability between the high- and low-spin states in spin-crossover materials provides a complex temperature dependence of the ordering processes. Thermodynamic properties of the ordering phenomena were studied in a unified way, and a generic structure of the ordering processes was proposed. The origin of the interaction among the spins was also discussed, and a new mechanism based on an elastic interaction among distortions due to the volume of a molecule depending on its spin state was also proposed. With this mechanism, the typical pressure dependence of the ordering processes can be reproduced. Moreover, we studied the type of criticality of the phase transition and pointed out that the present model possesses critical behaviour belonging to the mean-field universality class. There, the spin-spin correlation function is constant at long distances and does not show an exponential decay in contrast to short-range models. It is also pointed out that the model with periodic boundary conditions does not show ordering clusters, even near the critical point or in the process of spinodal decomposition. This indicates that critical opalescence would not be observed in this model. No cluster appears, either in photo-excitation process from the low-spin state at low temperatures. On the other hand, with open boundary conditions, the system shows a cluster structure. The effects of the boundary conditions are also discussed.

Rigorous spin-spin correlation function of Ising model on a special kind of Sierpinski Carpets

International Nuclear Information System (INIS)

Yang, Z.R.

1993-10-01

We have exactly calculated the rigorous spin-spin correlation function of Ising model on a special kind of Sierpinski Carpets (SC's) by means of graph expansion and a combinatorial approach and investigated the asymptotic behaviour in the limit of long distance. The result show there is no long range correlation between spins at any finite temperature which indicates no existence of phase transition and thus finally confirms the conclusion produced by the renormalization group method and other physical arguments. (author). 7 refs, 6 figs

Reorienting Hypnosis Education.

Science.gov (United States)

Alter, David S; Sugarman, Laurence Irwin

2017-01-01

The legacy model of professional clinical hypnosis training presents a restrictive frame increasingly incompatible with our evolving understanding of psychobiology, health, and care. Emerging science recognizes human experience not as disease and diagnosis, but as manifestations of individual, uniquely-endowed, adaptively self-regulating systems. Hypnosis is a particularly well-suited discipline for effecting beneficial change in this paradigm. Training in clinical hypnosis must progress from the current linearly-structured, diagnosis-based, reductionist model toward a more responsive, naturalistic, and client-centered curriculum in order to remain relevant and accessible to clinicians beginning to integrate it into their practices. To that end, this article extends Hope and Sugarman's (2015) thesis of hypnosis as a skill set for systemic perturbation and reorientation to consider what those skills may be, the principles on which they are based, and how they may be taught. Parsing a clinical vignette reveals how incorporation of novelty and uncertainty results in less restrictive and more naturalistic hypnotic encounters that, in response to client-generated cues, elicit psychophysiological plasticity. This disruptive hypnosis education and training framework extends the utility and benefit of applied clinical hypnosis.

A parity-breaking electronic nematic phase transition in the spin-orbit coupled correlated metal Cd2Re2O7

Science.gov (United States)

Harter, J. W.; Zhao, Z. Y.; Yan, J.-Q.; Mandrus, D. G.; Hsieh, D.

Strong interactions between electrons are known to drive metallic systems toward a variety of well-known symmetry-broken phases, including superconducting, electronic liquid crystalline, and charge- and spin-density wave ordered states. In contrast, the electronic instabilities of correlated metals with strong spin-orbit coupling have only recently begun to be explored. We uncover a novel multipolar nematic phase of matter in the metallic pyrochlore Cd2Re2O7 using spatially-resolved second-harmonic optical anisotropy measurements. Like previously discovered electronic liquid crystalline phases, this multipolar nematic phase spontaneously breaks rotational symmetry while preserving translational invariance. However, it has the distinguishing property of being odd under spatial inversion, which is allowed only in the presence of spin-orbit coupling. By examining the critical behavior of the multipolar nematic order parameter, we show that it drives the thermal phase transition near 200 K in Cd2Re2O7 and induces a parity-breaking lattice distortion as a secondary order parameter.

Surface-environment effects in spin crossover solids

Energy Technology Data Exchange (ETDEWEB)

Gudyma, Iu., E-mail: yugudyma@gmail.com; Maksymov, A.

2017-06-15

Highlights: • The spin-crossover nanocrystals were described by modified Ising-like model. • The ligand field on the surface is a function of external fluctuations. • The thermal hysteresis with surface and bulk interactions of the lattice was studied. • The system behavior with fluctuating ligand field on the surface was examined. • The fluctuations enlarge the hysteresis, but smaller surface interaction narrows it. - Abstract: The impact of surface effects on thermal induced spin crossover phenomenon is a subject of a broad and current interest. Using the modified Ising-like model of spin crossover solids with the ligand field as function of the molecule’ positions and random component on surface by means of Metropolis Monte Carlo algorithm the thermal spin transition curves were calculated. The analysis of spin configuration during transition gives a general idea about contribution of molecules from the surface and inside the lattice into resulting magnetization of the systems. The behavior of hysteresis loop for various surface coupling and fluctuations strength has been described.

Dynamic compensation temperatures in a mixed spin-1 and spin-3/2 Ising system under a time-dependent oscillating magnetic field

Energy Technology Data Exchange (ETDEWEB)

Keskin, Mustafa, E-mail: keskin@erciyes.edu.t [Department of Physics, Erciyes University, 38039 Kayseri (Turkey); Kantar, Ersin [Institute of Science, Erciyes University, 38039 Kayseri (Turkey)

2010-09-15

We study the existence of dynamic compensation temperatures in the mixed spin-1 and spin-3/2 Ising ferrimagnetic system Hamiltonian with bilinear and crystal-field interactions in the presence of a time-dependent oscillating external magnetic field on a hexagonal lattice. We employ the Glauber transitions rates to construct the mean-field dynamic equations. We investigate the time dependence of an average sublattice magnetizations, the thermal behavior of the dynamic sublattice magnetizations and the total magnetization. From these studies, we find the phases in the system, and characterize the nature (continuous or discontinuous) of transitions as well as obtain the dynamic phase transition (DPT) points and the dynamic compensation temperatures. We also present dynamic phase diagrams, including the compensation temperatures, in the five different planes. A comparison is made with the results of the available mixed spin Ising systems.

Dynamic compensation temperatures in a mixed spin-1 and spin-3/2 Ising system under a time-dependent oscillating magnetic field

International Nuclear Information System (INIS)

Keskin, Mustafa; Kantar, Ersin

2010-01-01

We study the existence of dynamic compensation temperatures in the mixed spin-1 and spin-3/2 Ising ferrimagnetic system Hamiltonian with bilinear and crystal-field interactions in the presence of a time-dependent oscillating external magnetic field on a hexagonal lattice. We employ the Glauber transitions rates to construct the mean-field dynamic equations. We investigate the time dependence of an average sublattice magnetizations, the thermal behavior of the dynamic sublattice magnetizations and the total magnetization. From these studies, we find the phases in the system, and characterize the nature (continuous or discontinuous) of transitions as well as obtain the dynamic phase transition (DPT) points and the dynamic compensation temperatures. We also present dynamic phase diagrams, including the compensation temperatures, in the five different planes. A comparison is made with the results of the available mixed spin Ising systems.

Pressure response of vacancy ordered maghemite (γ-Fe2O3) and high pressure transformed hematite (α-Fe2O3)

Science.gov (United States)

Hearne, Giovanni; Pischedda, Vittoria

2012-03-01

Combined XRD and Mössbauer effect spectroscopy studies to high pressures of ˜30 GPa of vacancy ordered maghemite are presented. The vacancy ordered superstructure is robust and remains intact up to the pressure-induced onset transition to hematite at 13-16 GPa. The pressure transformed hematite is shown to be crystallographically textured, unlike the randomised low pressure maghemite phase. This arises out of a pressure or stress instigated topotactic transformation of the cubic-spinel to hexagonal-corundum structure. The textured sample permits us to obtain information on the spin reorientation behavior of the pressure transformed hematite in compression and decompression sequences. Spin reorientation is restricted to ˜15° over wide pressure ranges, attributable to the effect of entrapped vacancies in the high pressure structure. Thus there are structural and magnetic peculiarities specific to pressure transformed hematite not evident in pressurized hematite starting material. These are triggered by the maghemite→hematite transformation.

Dynamical instability of a spin spiral in an interacting Fermi gas as a probe of the Stoner transition

Science.gov (United States)

Conduit, G. J.; Altman, E.

2010-10-01

We propose an experiment to probe ferromagnetic phenomena in an ultracold Fermi gas, while alleviating the sensitivity to three-body loss and competing many-body instabilities. The system is initialized in a small pitch spin spiral, which becomes unstable in the presence of repulsive interactions. To linear order the exponentially growing collective modes exhibit critical slowing down close to the Stoner transition point. Also, to this order, the dynamics are identical on the paramagnetic and ferromagnetic sides of the transition. However, we show that scattering off the exponentially growing modes qualitatively alters the collective mode structure. The critical slowing down is eliminated and in its place a new unstable branch develops at large wave vectors. Furthermore, long-wavelength instabilities are quenched on the paramagnetic side of the transition. We study the experimental observation of the instabilities, specifically addressing the trapping geometry and how phase-contrast imaging will reveal the emerging domain structure. These probes of the dynamical phenomena could allow experiments to detect the transition point and distinguish between the paramagnetic and ferromagnetic regimes.

Dynamical instability of a spin spiral in an interacting Fermi gas as a probe of the Stoner transition

International Nuclear Information System (INIS)

Conduit, G. J.; Altman, E.

2010-01-01

We propose an experiment to probe ferromagnetic phenomena in an ultracold Fermi gas, while alleviating the sensitivity to three-body loss and competing many-body instabilities. The system is initialized in a small pitch spin spiral, which becomes unstable in the presence of repulsive interactions. To linear order the exponentially growing collective modes exhibit critical slowing down close to the Stoner transition point. Also, to this order, the dynamics are identical on the paramagnetic and ferromagnetic sides of the transition. However, we show that scattering off the exponentially growing modes qualitatively alters the collective mode structure. The critical slowing down is eliminated and in its place a new unstable branch develops at large wave vectors. Furthermore, long-wavelength instabilities are quenched on the paramagnetic side of the transition. We study the experimental observation of the instabilities, specifically addressing the trapping geometry and how phase-contrast imaging will reveal the emerging domain structure. These probes of the dynamical phenomena could allow experiments to detect the transition point and distinguish between the paramagnetic and ferromagnetic regimes.

Dynamic phase transitions and dynamic phase diagrams of the spin-2 Blume-Capel model under an oscillating magnetic field within the effective-field theory

Energy Technology Data Exchange (ETDEWEB)

Ertas, Mehmet [Department of Physics, Erciyes University, 38039 Kayseri (Turkey); Institute of Science, Erciyes University, 38039 Kayseri (Turkey); Deviren, Bayram [Department of Physics, Nevsehir University, 50300 Nevsehir (Turkey); Keskin, Mustafa, E-mail: keskin@erciyes.edu.tr [Department of Physics, Erciyes University, 38039 Kayseri (Turkey)

2012-03-15

The dynamic phase transitions are studied in the kinetic spin-2 Blume-Capel model under a time-dependent oscillating magnetic field using the effective-field theory with correlations. The effective-field dynamic equation for the average magnetization is derived by employing the Glauber transition rates and the phases in the system are obtained by solving this dynamic equation. The nature (first- or second-order) of the dynamic phase transition is characterized by investigating the thermal behavior of the dynamic magnetization and the dynamic phase transition temperatures are obtained. The dynamic phase diagrams are constructed in the reduced temperature and magnetic field amplitude plane and are of seven fundamental types. Phase diagrams contain the paramagnetic (P), ferromagnetic-2 (F{sub 2}) and three coexistence or mixed phase regions, namely the F{sub 2}+P, F{sub 1}+P and F{sub 2}+F{sub 1}+P, which strongly depend on the crystal-field interaction (D) parameter. The system also exhibits the dynamic tricritical behavior. - Highlights: Black-Right-Pointing-Pointer Dynamic phase transitions are studied in spin-2 BC model using EFT. Black-Right-Pointing-Pointer Dynamic phase diagrams are constructed in (T/zJ, h/zJ) plane. Black-Right-Pointing-Pointer Seven fundamental types of dynamic phase diagrams are found in the system. Black-Right-Pointing-Pointer System exhibits dynamic tricritical behavior.

Re-orientating time in product design : a phenomenology-inspired perspective

NARCIS (Netherlands)

Stienstra, J.T.; Hengeveld, B.J.; Hummels, C.C.M.

2015-01-01

This paper presents a work in progress design case that is used to exemplify how a phenomenology-inspired perspective on time can impact the design of highly interactive systems and products. The design presents a calendar with a re-orientated layout that is based on a bodily relationship with time,

Stress-induced reorientation of hydride precipitates in Zr-2.5Nb-0.5Cu garter springs under complex loading

International Nuclear Information System (INIS)

De, P.K.; John, J.T.; Raman, V.V.; Banerjee, S.

1991-01-01

Zr-2.5Nb-0.5Cu garter springs which are placed between coolant and calandria tubes in PHWRs experience complex loading due to simultaneous application of tension, compression and torus bending moment due to coolant tubes. The gradual pick up of hydrogen by the garter springs during service is likely to have hydride platelets reoriented under the applied stresses. In the present paper, the magnitudes and the directions of the principal stresses under the complex loading condition obtained have been calculated and the extent of hydride reorientation predicted. Simulation experiments consisting of simulated loading of hydrogen (upto 400 ppm) precharged springs at the service temperature (300degC) and also in-situ hydrogen charging of the springs under simulated loading conditions have been carried out. In addition, hydrogen precharged springs have been subjected to temperature cycling between 50 and 300degC under complex loading conditions, to evaluate the influence of temperature variation on hydride reorientation. Metallographic examination of the hydride platelets in the above springs has shown an excellent agreement with the analytical prediction. Torus bending moment values appear to play a significant role in reorienting the hydride platelets. It has been observed that under normal torus bending moment corresponding to 90 mm dia coolant tubes hydrogen platelets close to the outer rim of the spiral get reoriented in the radial direction. However, on application a torus bending moment corresponding to 30 mm dia tubes, hydride platelets get reoriented along the radial direction, irrespective of the magnitude of tensile and compression loading. (author). 9 refs., 15 figs., 1 appendix

Bandwidth broadening and asymmetric softening of collective spin waves in magnonic crystals

International Nuclear Information System (INIS)

Montoncello, F.; Giovannini, L.

2014-01-01

We investigate the dependence on the applied field of the frequency/wavevector dispersion relations of collective spin waves in arrays of dots, close to a magnetic transition. In particular, we focus on the low frequency “soft” modes in three different cases: end modes in the transition between two different saturated states in ellipses, fundamental mode in the saturated-to-vortex transition in disks, and gyrotropic mode in the vortex-to-saturated transition in disks. Noteworthy, the spin waves with nonzero Bloch wavevector along the direction of the applied field happen to soften earlier than spin waves with a Bloch wavevector along different directions, and this feature is responsible for an asymmetric broadening of the bandwidth along the different lattice directions. This is particularly useful in magnonic/spin-logic device research, if different binary digits are associated to modes with the same cell function but different propagation directions.

Pure spin current manipulation in antiferromagnetically exchange coupled heterostructures

Science.gov (United States)

Avilés-Félix, L.; Butera, A.; González-Chávez, D. E.; Sommer, R. L.; Gómez, J. E.

2018-03-01

We present a model to describe the spin currents generated by ferromagnet/spacer/ferromagnet exchange coupled trilayer systems and heavy metal layers with strong spin-orbit coupling. By exploiting the magnitude of the exchange coupling (oscillatory RKKY-like coupling) and the spin-flop transition in the magnetization process, it has been possible to produce spin currents polarized in arbitrary directions. The spin-flop transition of the trilayer system originates pure spin currents whose polarization vector depends on the exchange field and the magnetization equilibrium angles. We also discuss a protocol to control the polarization sign of the pure spin current injected into the metallic layer by changing the initial conditions of magnetization of the ferromagnetic layers previously to the spin pumping and inverse spin Hall effect experiments. The small differences in the ferromagnetic layers lead to a change in the magnetization vector rotation that permits the control of the sign of the induced voltage components due to the inverse spin Hall effect. Our results can lead to important advances in hybrid spintronic devices with new functionalities, particularly, the ability to control microscopic parameters such as the polarization direction and the sign of the pure spin current through the variation of macroscopic parameters, such as the external magnetic field or the thickness of the spacer in antiferromagnetic exchange coupled systems.

Numerical Evidence for a Phase Transition in 4D Spin-Foam Quantum Gravity.

Science.gov (United States)

Bahr, Benjamin; Steinhaus, Sebastian

2016-09-30

Building on recent advances in defining Wilsonian renormalization group (RG) flows, and the notion of scales in particular, for background-independent theories, we present a first investigation of the renormalization of the 4D spin-foam path integral for quantum gravity, both analytically and numerically. Focusing on a specific truncation of the model using a hypercubic lattice, we compute the RG flow and find strong indications for a phase transition, as well as an interesting interplay between the different observed phases and the (broken) diffeomorphism symmetry of the model. Most notably, it appears that the critical point between the phases, which is a fixed point of the RG flow, is precisely where broken diffeomorphism symmetry is restored, which suggests that it might allow us to define a continuum limit of the quantum gravity theory.

Numerical Evidence for a Phase Transition in 4D Spin-Foam Quantum Gravity

Science.gov (United States)

Bahr, Benjamin; Steinhaus, Sebastian

2016-09-01

Building on recent advances in defining Wilsonian renormalization group (RG) flows, and the notion of scales in particular, for background-independent theories, we present a first investigation of the renormalization of the 4D spin-foam path integral for quantum gravity, both analytically and numerically. Focusing on a specific truncation of the model using a hypercubic lattice, we compute the RG flow and find strong indications for a phase transition, as well as an interesting interplay between the different observed phases and the (broken) diffeomorphism symmetry of the model. Most notably, it appears that the critical point between the phases, which is a fixed point of the RG flow, is precisely where broken diffeomorphism symmetry is restored, which suggests that it might allow us to define a continuum limit of the quantum gravity theory.

Spin polarized and density modulated phases in symmetric electron-electron and electron-hole bilayers.

Science.gov (United States)

Kumar, Krishan; Moudgil, R K

2012-10-17

We have studied symmetric electron-electron and electron-hole bilayers to explore the stable homogeneous spin phase and the feasibility of inhomogeneous charge-/spin-density ground states. The former is resolved by comparing the ground-state energies in states of different spin polarizations, while the latter is resolved by searching for a divergence in the wavevector-dependent static charge/spin susceptibility. For this endeavour, we have used the dielectric approach within the self-consistent mean-field theory of Singwi et al. We find that the inter-layer interactions tend to change an abrupt spin-polarization transition of an isolated layer into a nearly gradual one, even though the partially spin-polarized phases are not clearly stable within the accuracy of our calculation. The transition density is seen to decrease with a reduction in layer spacing, implying a suppression of spin polarization by inter-layer interactions. Indeed, the suppression shows up distinctly in the spin susceptibility computed from the spin-polarization dependence of the ground-state energy. However, below a critical layer spacing, the unpolarized liquid becomes unstable against a charge-density-wave (CDW) ground state at a density preceding full spin polarization, with the transition density for the CDW state increasing on further reduction in the layer spacing. Due to attractive e-h correlations, the CDW state is found to be more pronounced in the e-h bilayer. On the other hand, the static spin susceptibility diverges only in the long-wavelength limit, which simply represents a transition to the homogeneous spin-polarized phase.

Electric-field effects in optically generated spin transport

International Nuclear Information System (INIS)

Miah, M. Idrish

2009-01-01

Transport of spin-polarized electrons in semiconductors is studied experimentally. Spins are generated by optical excitation because of the selection rules governing optical transitions from heavy-hole and light-hole states to conduction-band states. Experiments designed for the control of spins in semiconductors investigate the bias-dependent spin transport process and detect the spin-polarized electrons during transport. A strong bias dependence is observed. The electric-field effects on the spin-polarized electron transport are also found to be depended on the excitation photon energy and temperature. Based on a field-dependent spin relaxation mechanism, the electric-field effects in the transport process are discussed.

Electric-field effects in optically generated spin transport

Energy Technology Data Exchange (ETDEWEB)

Miah, M. Idrish [Nanoscale Science and Technology Centre and School of Biomolecular and Physical Sciences, Griffith University, Nathan, Brisbane, QLD 4111 (Australia); Department of Physics, University of Chittagong, Chittagong 4331 (Bangladesh)], E-mail: m.miah@griffith.edu.au

2009-05-25

Transport of spin-polarized electrons in semiconductors is studied experimentally. Spins are generated by optical excitation because of the selection rules governing optical transitions from heavy-hole and light-hole states to conduction-band states. Experiments designed for the control of spins in semiconductors investigate the bias-dependent spin transport process and detect the spin-polarized electrons during transport. A strong bias dependence is observed. The electric-field effects on the spin-polarized electron transport are also found to be depended on the excitation photon energy and temperature. Based on a field-dependent spin relaxation mechanism, the electric-field effects in the transport process are discussed.

Coupling a Surface Acoustic Wave to an Electron Spin in Diamond via a Dark State

Directory of Open Access Journals (Sweden)

D. Andrew Golter

2016-12-01

Full Text Available The emerging field of quantum acoustics explores interactions between acoustic waves and artificial atoms and their applications in quantum information processing. In this experimental study, we demonstrate the coupling between a surface acoustic wave (SAW and an electron spin in diamond by taking advantage of the strong strain coupling of the excited states of a nitrogen vacancy center while avoiding the short lifetime of these states. The SAW-spin coupling takes place through a Λ-type three-level system where two ground spin states couple to a common excited state through a phonon-assisted as well as a direct dipole optical transition. Both coherent population trapping and optically driven spin transitions have been realized. The coherent population trapping demonstrates the coupling between a SAW and an electron spin coherence through a dark state. The optically driven spin transitions, which resemble the sideband transitions in a trapped-ion system, can enable the quantum control of both spin and mechanical degrees of freedom and potentially a trapped-ion-like solid-state system for applications in quantum computing. These results establish an experimental platform for spin-based quantum acoustics, bridging the gap between spintronics and quantum acoustics.

Ordering phenomena in transition-metal-oxide heterostructures

Energy Technology Data Exchange (ETDEWEB)

Frano Pereira, Alex Manuel

2014-01-27

This doctoral work presents a study of ordered ground states of transition metal oxide compounds and multilayers using resonant elastic soft x-ray scattering. The technique has developed over the last decades and become especially useful when sample sizes are limited like the case of nanometer-scale films and superlattices. By scattering with photon energies on resonance with the element's electronic transitions, it is an element-specific, sensitive tool providing a combination of spectroscopic and spatial information. The thesis is divided into two central topics. The first part focuses on the investigation of perovskite-type, rare-earth nickelate heterostructures. X-rays tuned to the Ni L{sub 3}-edge were used to unveil unprecedented diffraction evidence of long range magnetic order in LaNiO{sub 3}-RXO{sub 3} (RXO{sub 3} = LaAlO{sub 3}, DyScO{sub 3}) superlattices. We report on the appearance of magnetic order in such systems with a propagation vector of Q{sub SDW} = ((1)/(4),(1)/(4),l) in pseudocubic notation, similar to bulk rare earth nickelates with R ≠ La. With LaNiO{sub 3} being paramagnetic in its bulk form, the magnetic Bragg peak is only present in superlattices where the thickness of the LaNiO{sub 3} layers approaches the 2-dimensional limit. Besides the thickness dependence, the magnetic order was probed on samples grown on varying strain-inducing substrates. Azimuthal scans around Q{sub SDW} were done to determine the orientation of the spin spiral under these different conditions. We will explain how the reorientation of the spins can be understood by the magneto-crystalline anisotropy which is determined by the relative occupation of the Ni d-orbitals via spin-orbit coupling. First steps towards control of the spin spiral's orientation will be outlined, and along with the high remanent conductivity found in the magnetic spiral state, an outlook for metallic antiferromagnetic spintronics will be discussed. The second part of this thesis

Spin-flip effects on the supercurrent through mesoscopic superconducting junctions

International Nuclear Information System (INIS)

Pan Hui; Lin Tsunghan

2005-01-01

We investigate the spin-flip effects on the Andreev bound states and the supercurrent in a superconductor/quantum-dot/superconductor system, theoretically. The spin-flip scattering in the quantum dot can reverse the supercurrent flowing through the system, which results in a π-junction transition. By controlling the energy level of the quantum dot, the π-junction transition can be caused to occur again. The two mechanisms of the π-junction transitions are interpreted within the picture of Andreev bound states

One and two-phonon processes of the spin-flip relaxation in quantum dots: Spin-phonon coupling mechanism

Science.gov (United States)

Wang, Zi-Wu; Li, Shu-Shen

2012-07-01

We investigate the spin-flip relaxation in quantum dots using a non-radiation transition approach based on the descriptions for the electron-phonon deformation potential and Fröhlich interaction in the Pavlov-Firsov spin-phonon Hamiltonian. We give the comparisons of the electron relaxations with and without spin-flip assisted by one and two-phonon processes. Calculations are performed for the dependence of the relaxation time on the external magnetic field, the temperature and the energy separation between the Zeeman sublevels of the ground and first-excited state. We find that the electron relaxation time of the spin-flip process is more longer by three orders of magnitudes than that of no spin-flip process.

Reorientational motion of a cross-link junction in a poly(dimethylsiloxane) network measured by time-resolved fluorescence depolarization

Energy Technology Data Exchange (ETDEWEB)

Stein, A.D. (Department of Chemistry, Stanford University, Stanford, California 94305 (United States)); Hoffman, D.A. (Department of Materials Science and Engineering, Stanford University, Stanford, California 94305 (United States)); Frank, C.W. (Department of Chemical Engineering, Stanford University, Stanford, California 94305 (United States)); Fayer, M.D. (Department of Chemistry, Stanford University, Stanford, California 94305 (United States))

1992-02-15

The reorientational dynamics of a cross-link junction in poly(dimethylsiloxane) networks, measured by the fluorescence anisotropy decay of a chromophore tagged to the cross-link, have been investigated over a range of temperatures from {ital T}{sub {ital g}}+75 to {ital T}{sub {ital g}}+150. The probe chromophore, 1-dimethylamino-5-sulfonylnaphthalene amide (dansyl amide), is pendant to a trifunctional silane that acts as a cross-linking molecule. In cyclohexanol, the fluorescence anisotropy decay is in agreement with Debye--Stokes--Einstein hydrodynamic theory (rotational diffusion) demonstrating that the cross-linker can be used as a probe of orientational relaxation. The fluorescence anisotropy decays at a rapid rate in an end-linked poly(dimethyl siloxane) network reflecting fast reorientational motion of the cross-link junction. This reorientation appears diffusive and has a temperature dependence in accord with the Williams--Landel--Ferry equation. A model is proposed that suggests that reorientation and translational motion of the cross-link occur simultaneously and are both coupled to fluctuations of the polymer chain ends.

Transition probability spaces in loop quantum gravity

Science.gov (United States)

Guo, Xiao-Kan

2018-03-01

We study the (generalized) transition probability spaces, in the sense of Mielnik and Cantoni, for spacetime quantum states in loop quantum gravity. First, we show that loop quantum gravity admits the structures of transition probability spaces. This is exemplified by first checking such structures in covariant quantum mechanics and then identifying the transition probability spaces in spin foam models via a simplified version of general boundary formulation. The transition probability space thus defined gives a simple way to reconstruct the discrete analog of the Hilbert space of the canonical theory and the relevant quantum logical structures. Second, we show that the transition probability space and in particular the spin foam model are 2-categories. Then we discuss how to realize in spin foam models two proposals by Crane about the mathematical structures of quantum gravity, namely, the quantum topos and causal sites. We conclude that transition probability spaces provide us with an alternative framework to understand various foundational questions of loop quantum gravity.

Voltage control of magnetic monopoles in artificial spin ice

Science.gov (United States)

Chavez, Andres C.; Barra, Anthony; Carman, Gregory P.

2018-06-01

Current research on artificial spin ice (ASI) systems has revealed unique hysteretic memory effects and mobile quasi-particle monopoles controlled by externally applied magnetic fields. Here, we numerically demonstrate a strain-mediated multiferroic approach to locally control the ASI monopoles. The magnetization of individual lattice elements is controlled by applying voltage pulses to the piezoelectric layer resulting in strain-induced magnetic precession timed for 180° reorientation. The model demonstrates localized voltage control to move the magnetic monopoles across lattice sites, in CoFeB, Ni, and FeGa based ASI’s. The switching is achieved at frequencies near ferromagnetic resonance and requires energies below 620 aJ. The results demonstrate that ASI monopoles can be efficiently and locally controlled with a strain-mediated multiferroic approach.

Detecting the multi-spin interaction of an XY spin chain by the geometric phase of a coupled qubit

International Nuclear Information System (INIS)

Zhang, Xiu-xing; Zhang, Ai-ping; Li, Fu-li

2012-01-01

We investigate geometric phase (GP) of a qubit symmetrically coupled to a XY spin chain with three-spin interaction in a transverse magnetic field. An analytical expression for the GP is found in the weak coupling limit. It is shown that the GP displays a sharp peak or dip around the quantum phase transition point of the spin chain. Without the three-spin interaction, the GP has a peak or dip around the critical point λ=1. If the three-spin interaction exists, the peak or dip position is obviously shifted away from the original position. This result reveals that the GP may be taken as an observable to detect both the existence and strength of multi-spin interaction in a spin chain. -- Highlights: ► Analytical expression for geometric phase (GP) of a qubit coupled to a spin chain is obtained. ► Relation between GP and multi-spin interaction is investigated. ► Detection of multi-spin interaction by means of GP is proposed.

Characteristics of hydride precipitation and reorientation in spent-fuel cladding

International Nuclear Information System (INIS)

Chung, H. M.; Strain, R. V.; Billone, M. C.

2000-01-01

The morphology, number density, orientation, distribution, and crystallographic aspects of Zr hydrides in Zircaloy fuel cladding play important roles in fuel performance during all phases before and after discharge from the reactor, i.e., during normal operation, transient and accident situations in the reactor, temporary storage in a dry cask, and permanent storage in a waste repository. In the past, partly because of experimental difficulties, hydriding behavior in irradiated fuel cladding has been investigated mostly by optical microscopy (OM). In the present study, fundamental metallurgical and crystallographic characteristics of hydride precipitation and reorientation were investigated on the microscopic level by combined techniques of OM and transmission electron and scanning electron microscopy (TEM and SEM) of spent-fuel claddings discharged from several boiling and pressurized water reactors (BWRs and PWRs). Defueled sections of standard and Zr-lined Zircaloy-2 fuel claddings, irradiated to fluences of ∼3.3 x 10 21 n cm -2 and ∼9.2 x 10 21 n cm -2 (E > 1 MeV), respectively, were obtained from spent fuel rods discharged from two BWRs. Sections of standard and low-tin Zircaloy-4 claddings, irradiated to fluences of ∼4.4 x 10 21 n cm -2 , ∼5.9 x 10 21 n cm -2 , and ∼9.6 x 10 21 n cm -2 (E > 1 MeV) in three PWRs, were also obtained. Microstructural characteristics of hydrides were analyzed in as-irradiated condition and after gas-pressurization-burst or expanding-mandrel tests at 292-325 C in Ar for some of the spent-fuel claddings. Analyses were also conducted of hydride habit plane, morphology, and reorientation characteristics on unirradiated Zircaloy-4 cladding that contained dense radial hydrides. Reoriented hydrides in the slowly cooled unirradiated cladding were produced by expanding-mandrel loading

Anisotropic optical absorption induced by Rashba spin-orbit coupling in monolayer phosphorene

Science.gov (United States)

Li, Yuan; Li, Xin; Wan, Qi; Bai, R.; Wen, Z. C.

2018-04-01

We obtain the effective Hamiltonian of the phosphorene including the effect of Rashba spin-orbit coupling in the frame work of the low-energy theory. The spin-splitting energy bands show an anisotropy feature for the wave vectors along kx and ky directions, where kx orients to ΓX direction in the k space. We numerically study the optical absorption of the electrons for different wave vectors with Rashba spin-orbit coupling. We find that the spin-flip transition from the valence band to the conduction band induced by the circular polarized light closes to zero with increasing the x-component wave vector when ky equals to zero, while it can be significantly increased to a large value when ky gets a small value. When the wave vector varies along the ky direction, the spin-flip transition can also increase to a large value, however, which shows an anisotropy feature for the optical absorption. Especially, the spin-conserved transitions keep unchanged and have similar varying trends for different wave vectors. This phenomenon provides a novel route for the manipulation of the spin-dependent property of the fermions in the monolayer phosphorene.

Spin correlations in quantum wires

Science.gov (United States)

Sun, Chen; Pokrovsky, Valery L.

2015-04-01

We consider theoretically spin correlations in a one-dimensional quantum wire with Rashba-Dresselhaus spin-orbit interaction (RDI). The correlations of noninteracting electrons display electron spin resonance at a frequency proportional to the RDI coupling. Interacting electrons, upon varying the direction of the external magnetic field, transit from the state of Luttinger liquid (LL) to the spin-density wave (SDW) state. We show that the two-time total-spin correlations of these states are significantly different. In the LL, the projection of total spin to the direction of the RDI-induced field is conserved and the corresponding correlator is equal to zero. The correlators of two components perpendicular to the RDI field display a sharp electron-spin resonance driven by the RDI-induced intrinsic field. In contrast, in the SDW state, the longitudinal projection of spin dominates, whereas the transverse components are suppressed. This prediction indicates a simple way for an experimental diagnostic of the SDW in a quantum wire. We point out that the Luttinger model does not respect the spin conservation since it assumes the infinite Fermi sea. We propose a proper cutoff to correct this failure.

Nuclear spin bath effects in molecular nanomagnets: Direct quantum mechanical simulations

Science.gov (United States)

Sinitsyn, N. A.; Dobrovitski, V. V.

2004-11-01

We investigate the influence of nuclear spins on the electronic spin tunneling in magnetic molecules such as Fe8 , focusing on the role of the spin diffusion in the nuclear spin bath. We simulate the quantum spin dynamics by numerically solving the time-dependent Schrödinger equation for the compound system (the electronic spin plus the bath spins). Our results demonstrate that the effect of the spin bath cannot always be modeled as a randomly varying magnetic field acting on the electronic spin. We consider two dynamical regimes: the spin relaxation in a constant magnetic field, and the spin tunneling in the linearly varying magnetic field passing the avoided level crossing, so-called Landau-Zener-Stückelberg (LZS) transition. For the first regime, we confirmed that the hole in the magnetization distribution has the width of the hyperfine fields distribution. For the second regime, we found that the transition probability for moderately slow sweeps deviates from the standard LZS prediction, while for the fast sweeps the deviation is negligible.

Effects of hydrostatic pressure and uniaxial strain on spin-Peierls transition in an organic radical magnet, BBDTA·InCl4

International Nuclear Information System (INIS)

Mito, Masaki; Kawagoe, Seiichiro; Deguchi, Hiroyuki; Takagi, Seichi; Fujita, Wataru; Awaga, Kunio; Kondo, Ryusuke; Kagoshima, Seiichi

2009-01-01

We investigated the effects of hydrostatic pressure and uniaxial strain on the spin-Peierls (SP) transition of an organic radical magnet, benzo[1,2-d:4,5-d']bis[1,3,2]dithiazole(BBDTA)·InCl 4 . It has a one-dimensional coordination polymer structure along its c-axis and its SP transition occurs at 108 K. The SP transition temperature T SP decreased to 99 K at a hydrostatic pressure of 10 kbar, while it increased to 132 K at a uniaxial strain along the c-axis of 8 kbar. The pressure dependences of T SP under these two conditions were discussed by evaluating two parameters, namely, the intrachain interaction 2J/k B and the effective spin-lattice coupling parameter η, that are related to T SP by the equation T SP =1.6ηJ/k B . Under ambient pressure, the a- and c-axes of this material shortened monotonically with decreasing temperature, while the b-axis elongated below T SP . In this study, we found the correlation between η and the change in the lattice constant b. 2J/k B increased with increasing hydrostatic pressure and uniaxial strain, suggesting that the contraction along the c-axis does not depend on the manner of pressurization. From the evaluation of η, the observed variation in T SP is explained by the difference between the changes in b under the two pressurization conditions. (author)

Magnetic transitions and phases in random-anisotropy magnets

International Nuclear Information System (INIS)

Sellmyer, D.J.; Nafis, S.; O'Shea, M.J.

1988-01-01

The generality and universality of the Ising spin-glass-like phase transitions observed in several rare-earth, random-anisotropy magnets are discussed. Some uncertainties and practical problems in determining critical exponents are considered, and a comparison is made to insulating spin glasses and crystalline spin glasses where an apparent anisotropy-induced crossover from Heisenberg to Ising-like behavior is seen. The observation of a reentrant transition in a weak anisotropy system and its correlation with the theory of Chudnovsky, Saslow, and Serota [Phys. Rev. B 33, 251 (1986)] for the correlated spin glass is discussed

Magnetic transitions and phases in random-anisotropy magnets

Science.gov (United States)

Sellmyer, D. J.; Nafis, S.; O'Shea, M. J.

1988-04-01

The generality and universality of the Ising spin-glass-like phase transitions observed in several rare-earth, random-anisotropy magnets are discussed. Some uncertainties and practical problems in determining critical exponents are considered, and a comparison is made to insulating spin glasses and crystalline spin glasses where an apparent anisotropy-induced crossover from Heisenberg to Ising-like behavior is seen. The observation of a reentrant transition in a weak anisotropy system and its correlation with the theory of Chudnovsky, Saslow, and Serota [Phys. Rev. B 33, 251 (1986)] for the correlated spin glass is discussed.

Spin interferometry and phase relations in three level systems

International Nuclear Information System (INIS)

Mehring, M.; Stoll, M.E.; Wolff, E.K.

1978-01-01

The sign of the wavefunctions of deuterium, a spin-1 nucleus, under a 2π rotation (spinor character) has been studied with using a single crystal of 98% deuterated hexamethyl-benzene (HMB, C 6 (CD 3 ) 6 ). In a large magnetic fields, the three energy levels of the Zeeman hamiltonian have equal spacing, whereas unequivalent transition frequencies may occur if a suitable quadrupolar interaction is included. Three types of experiment are discussed. Simultaneous irradiation of both transitions with a field strength ω 1 in the x direction verified spin-locking, quadrature, or phase variation; consecutive irradiation at both transition with π-pulses showed coherence transfer from transition 1-2 to the forbidden transition 1-3; double quantum spinor behavior was demonstrated by applying rf field of strength ω 1 = γH 1 at the 'double quantum transition' frequency ω 0

Creating Spin-One Fermions in the Presence of Artificial Spin-Orbit Fields: Emergent Spinor Physics and Spectroscopic Properties

Science.gov (United States)

Kurkcuoglu, Doga Murat; de Melo, C. A. R. Sá

2018-05-01

We propose the creation and investigation of a system of spin-one fermions in the presence of artificial spin-orbit coupling, via the interaction of three hyperfine states of fermionic atoms to Raman laser fields. We explore the emergence of spinor physics in the Hamiltonian described by the interaction between light and atoms, and analyze spectroscopic properties such as dispersion relation, Fermi surfaces, spectral functions, spin-dependent momentum distributions and density of states. Connections to spin-one bosons and SU(3) systems is made, as well relations to the Lifshitz transition and Pomeranchuk instability are presented.

Field-induced negative differential spin lifetime in silicon.

Science.gov (United States)

Li, Jing; Qing, Lan; Dery, Hanan; Appelbaum, Ian

2012-04-13

We show that the electric-field-induced thermal asymmetry between the electron and lattice systems in pure silicon substantially impacts the identity of the dominant spin relaxation mechanism. Comparison of empirical results from long-distance spin transport devices with detailed Monte Carlo simulations confirms a strong spin depolarization beyond what is expected from the standard Elliott-Yafet theory even at low temperatures. The enhanced spin-flip mechanism is attributed to phonon emission processes during which electrons are scattered between conduction band valleys that reside on different crystal axes. This leads to anomalous behavior, where (beyond a critical field) reduction of the transit time between spin-injector and spin-detector is accompanied by a counterintuitive reduction in spin polarization and an apparent negative spin lifetime.

Entanglement and quantum phase transitions in matrix-product spin-1 chains

International Nuclear Information System (INIS)

Alipour, S.; Karimipour, V.; Memarzadeh, L.

2007-01-01

We consider a one-parameter family of matrix-product states of spin-1 particles on a periodic chain and study in detail the entanglement properties of such a state. In particular, we calculate exactly the entanglement of one site with the rest of the chain, and the entanglement of two distant sites with each other, and show that the derivative of both these properties diverge when the parameter g of the states passes through a critical point. Such a point can be called a point of quantum phase transition, since at this point the character of the matrix-product state, which is the ground state of a Hamiltonian, changes discontinuously. We also study the finite size effects and show how the entanglement depends on the size of the chain. This later part is relevant to the field of quantum computation where the problem of initial state preparation in finite arrays of qubits or qutrits is important. It is also shown that the entanglement of two sites have scaling behavior near the critical point

Intragranular twinning, detwinning, and twinning-like lattice reorientation in magnesium alloys

International Nuclear Information System (INIS)

Wu, Wei; Gao, Yanfei; Li, Nan; Parish, Chad M.; Liu, Wenjun; Liaw, Peter K.; An, Ke

2016-01-01

Deformation twinning plays a critical role on improving metals or alloys ductility, especially for hexagonal close-packed materials with low symmetry crystal structure. A rolled Mg alloy was selected as a model system to investigate the extension twinning behaviors and characteristics of parent-twin interactions by nondestructive in situ 3D synchrotron X-ray microbeam diffraction. Besides twinning-detwinning process, the “twinning-like” lattice reorientation process was captured within an individual grain inside a bulk material during the strain reversal. The distributions of parent, twin, and reorientated grains and sub-micron level strain variation across the twin boundary are revealed. A theoretical calculation of the lattice strain confirms that the internal strain distribution in parent and twinned grains correlates with the experimental setup, grain orientation of parent, twin, and surrounding grains, as well as the strain path changes. The study suggests a novel deformation mechanism within the hexagonal close-packed structure that cannot be determined from surface-based characterization methods.

Phase diagrams of a nonequilibrium mixed spin-3/2 and spin-2 Ising system in an oscillating magnetic field

International Nuclear Information System (INIS)

Keskin, Mustafa; Polat, Yasin

2009-01-01

The phase diagrams of the nonequilibrium mixed spin-3/2 and spin-2 Ising ferrimagnetic system on square lattice under a time-dependent external magnetic field are presented by using the Glauber-type stochastic dynamics. The model system consists of two interpenetrating sublattices of spins σ=3/2 and S=2, and we take only nearest-neighbor interactions between pairs of spins. The system is in contact with a heat bath at absolute temperature T abs and the exchange of energy with the heat bath occurs via one-spin flip of the Glauber dynamics. First, we investigate the time variations of average order parameters to find the phases in the system and then the thermal behavior of the dynamic order parameters to obtain the dynamic phase transition (DPT) points as well as to characterize the nature (first- or second-order) phase transitions. The dynamic phase diagrams are presented in two different planes. Phase diagrams contain paramagnetic (p), ferrimagnetic (i 1 , i 2 , i 3 ) phases, and three coexistence or mixed phase regions, namely i 1 +p, i 2 +p and i 3 +p mixed phases that strongly depend on interaction parameters.

Phase diagrams of a nonequilibrium mixed spin-3/2 and spin-2 Ising system in an oscillating magnetic field

Energy Technology Data Exchange (ETDEWEB)

Keskin, Mustafa [Department of Physics, Erciyes University, 38039 Kayseri (Turkey)], E-mail: keskin@erciyes.edu.tr; Polat, Yasin [Institutes of Science, Erciyes University, 38039 Kayseri (Turkey)

2009-12-15

The phase diagrams of the nonequilibrium mixed spin-3/2 and spin-2 Ising ferrimagnetic system on square lattice under a time-dependent external magnetic field are presented by using the Glauber-type stochastic dynamics. The model system consists of two interpenetrating sublattices of spins {sigma}=3/2 and S=2, and we take only nearest-neighbor interactions between pairs of spins. The system is in contact with a heat bath at absolute temperature T{sub abs} and the exchange of energy with the heat bath occurs via one-spin flip of the Glauber dynamics. First, we investigate the time variations of average order parameters to find the phases in the system and then the thermal behavior of the dynamic order parameters to obtain the dynamic phase transition (DPT) points as well as to characterize the nature (first- or second-order) phase transitions. The dynamic phase diagrams are presented in two different planes. Phase diagrams contain paramagnetic (p), ferrimagnetic (i{sub 1}, i{sub 2}, i{sub 3}) phases, and three coexistence or mixed phase regions, namely i{sub 1}+p, i{sub 2}+p and i{sub 3}+p mixed phases that strongly depend on interaction parameters.

Dual descriptors within the framework of spin-polarized density functional theory.

Science.gov (United States)

Chamorro, E; Pérez, P; Duque, M; De Proft, F; Geerlings, P

2008-08-14

Spin-polarized density functional theory (SP-DFT) allows both the analysis of charge-transfer (e.g., electrophilic and nucleophilic reactivity) and of spin-polarization processes (e.g., photophysical changes arising from electron transitions). In analogy with the dual descriptor introduced by Morell et al. [J. Phys. Chem. A 109, 205 (2005)], we introduce new dual descriptors intended to simultaneously give information of the molecular regions where the spin-polarization process linking states of different multiplicity will drive electron density and spin density changes. The electronic charge and spin rearrangement in the spin forbidden radiative transitions S(0)-->T(n,pi(*)) and S(0)-->T(pi,pi(*)) in formaldehyde and ethylene, respectively, have been used as benchmark examples illustrating the usefulness of the new spin-polarization dual descriptors. These quantities indicate those regions where spin-orbit coupling effects are at work in such processes. Additionally, the qualitative relationship between the topology of the spin-polarization dual descriptors and the vertical singlet triplet energy gap in simple substituted carbene series has been also discussed. It is shown that the electron density and spin density rearrangements arise in agreement with spectroscopic experimental evidence and other theoretical results on the selected target systems.

Quasiclassical Theory of Spin Dynamics in Superfluid ^3He: Kinetic Equations in the Bulk and Spin Response of Surface Majorana States

Science.gov (United States)

Silaev, M. A.

2018-06-01

We develop a theory based on the formalism of quasiclassical Green's functions to study the spin dynamics in superfluid ^3He. First, we derive kinetic equations for the spin-dependent distribution function in the bulk superfluid reproducing the results obtained earlier without quasiclassical approximation. Then, we consider spin dynamics near the surface of fully gapped ^3He-B-phase taking into account spin relaxation due to the transitions in the spectrum of localized fermionic states. The lifetimes of longitudinal and transverse spin waves are calculated taking into account the Fermi-liquid corrections which lead to a crucial modification of fermionic spectrum and spin responses.

Chiral-glass transition in a diluted dipolar-interaction Heisenberg system

International Nuclear Information System (INIS)

Zhang Kaicheng; Liu Guibin; Zhu Yan

2011-01-01

Recently, numerical simulations reveal that a spin-glass transition can occur in the three-dimensional diluted dipolar system. By defining the chirality of triple spins in a diluted dipolar Heisenberg spin glass, we study the chiral ordering in the system using parallel tempering algorithm and heat bath method. The finite-size scaling analysis reveals that the system undergoes a chiral-glass transition at finite temperature. - Highlights: → We define the chirality in a diluted dipolar Heisenberg system. → The system undergoes a chiral-glass transition at finite temperature. → We extract the critical exponents of the chiral-glass transition.

Spin-crossover behavior of polymeric iron(III) complexes

International Nuclear Information System (INIS)

Maeda, Yonezo; Miyamoto, Makoto; Takashima, Yoshimasa; Oshio, Hiroaki

1989-01-01

Polymeric spin-crossover iron(III) complexes possessing poly(4-vinylpyridine), poly(N-vinylimidazole) or poly(octylmethacrylate-co-4-vinylpyridine) as ligand are prepared. In this experience enriched 57 Fe was used to get strong Moessbauer absorption. The enriched behavior of the complexes were examined by magnetic susceptibilities measurement, and Moessbauer and esr spectroscopies. Some of them show spin-state behavior over a wide range of temperature. Some of them show rapid spin-state interexchange compared to the Moessbauer time scale and others not. Spin-crossover behavior of polymeric complexes is characterized of wide spin-state transition temperature range

Spin-flip transitions in self-assembled quantum dots

Science.gov (United States)

Stavrou, V. N.

2017-12-01

Detailed realistic calculations of the spin-flip time (T 1) for an electron in a self-assembled quantum dot (SAQD) due to emission of an acoustic phonon, using only bulk properties with no fitting parameters, are presented. Ellipsoidal lens shaped Inx Ga1-x As quantum dots, with electronic states calculated using 8-band strain dependent {k \\cdot p} theory, are considered. The phonons are treated as bulk acoustic phonons coupled to the electron by both deformation potential and piezoelectric interactions. The dependence of T 1 on the geometry of SAQD, on the applied external magnetic field and on the lattice temperature is highlighted. The theoretical results are close to the experimental measurements on the spin-flip times for a single electron in QD.

Spin and orbital moments in actinide compounds

DEFF Research Database (Denmark)

Lebech, B.; Wulff, M.; Lander, G.H.

1991-01-01

The extended spatial distribution of both the transition-metal 3d electrons and the actinide 5f electrons results in a strong interaction between these electron states when the relevant elements are alloyed. A particular interesting feature of this hybridization, which is predicted by single...... experiments designed to determine the magnetic moments at the actinide and transition-metal sublattice sites in compounds such as UFe2, NpCo2, and PuFe2 and to separate the spin and orbital components at the actinide sites. The results show, indeed, that the ratio of the orbital to spin moment is reduced...

Spin-flip transition and Faraday effect in antiferromagnet KMnF3 in megagauss magnetic field

International Nuclear Information System (INIS)

Mukhin, A.A.; Plis, V.I.; Popov, A.I.; Zvezdin, A.K.; Platonov, V.; Tatsenko, O.M.

1998-01-01

Faraday effect in the antiferromagnet KMnF 3 has been investigated in pulse explosive fields up to 500 T at T=78 K. The laser wavelength 0.63 μm was used in the experiment. The magnetic field dependence of Faraday rotation in this antiferromagnet shows a unique feature of a lack of saturation effect in the fields up to 500 T whereas critical field of spin-flip transition is about 120 T. The theoretical analysis of microscopic nature of Faraday rotation, including the diamagnetic, magneto-dipole and paramagnetic mechanisms has been performed. The strong competition of these mechanisms is important to explain the extremely small value of the effect and its unusual magnetic field dependence

Erratum to: Quadrupole moments of low-lying baryons with spin ...

Indian Academy of Sciences (India)

physics pp. 1083. Erratum to: Quadrupole moments of low-lying baryons with spin-. 1. 2. +. , spin-. 3. 2. +. , and spin-. 3. 2. +. → 1. 2. + transitions. NEETIKA SHARMA and HARLEEN DAHIYA. ∗. Department of Physics, Dr. B.R. Ambedkar National Institute of Technology,. Jalandhar 144 011, India. ∗. Corresponding author.

Sign rules for anisotropic quantum spin systems

International Nuclear Information System (INIS)

Bishop, R. F.; Farnell, D. J. J.; Parkinson, J. B.

2000-01-01

We present exact ''sign rules'' for various spin-s anisotropic spin-lattice models. It is shown that, after a simple transformation which utilizes these sign rules, the ground-state wave function of the transformed Hamiltonian is positive definite. Using these results exact statements for various expectation values of off-diagonal operators are presented, and transitions in the behavior of these expectation values are observed at particular values of the anisotropy. Furthermore, the importance of such sign rules in variational calculations and quantum Monte Carlo calculations is emphasized. This is illustrated by a simple variational treatment of a one-dimensional anisotropic spin model

Spin-state studies with XES and RIXS: From static to ultrafast