WorldWideScience

Sample records for short-lived fallout radionuclides

  1. Radiopharmaceuticals and other compounds labelled with short-lived radionuclides

    CERN Document Server

    Welch, Michael J

    2013-01-01

    Radiopharmaceuticals and Other Compounds Labelled with Short-Lived Radionuclides covers through both review and contributed articles the potential applications and developments in labeling with short-lived radionuclides whose use is restricted to institutions with accelerators. The book discusses the current and potential use of generator-produced radionuclides as well as other short-lived radionuclides, and the problems of quality control of such labeled compounds. The book is useful to nuclear medicine physicians.

  2. Activation analysis with neutron generators using short-lived radionuclides

    International Nuclear Information System (INIS)

    Salma, I.

    1993-01-01

    The short half-life involves a number of important differences in production, transportation and measurement of radionuclides, and in counting statistics as compared with those in traditional activation analysis. Experiments were performed to investigate the analytical possibilities and prospective utilization of short-lived radionuclides produced by 14-MeV neutron irradiation. A rapid pneumatic transfer system for use with neutron generators was installed and applied for detecting radionuclides with a half-life from 300 ms to 30 s. The transport time for samples with a total mass of 1-4 g is between 130 and 160 ms for pressurized air of 0.1-0.4 MPa. 11 elements were studied by the conventional activation method using both a typical pneumatic transport system (run time 3 s) and the fast pneumatic transport facility. The effect of the cyclic activation technique on the elemental sensitivities was also investigated. (orig.)

  3. Production of medical short-lived radionuclides in Canada

    International Nuclear Information System (INIS)

    Wiebe, L.I.

    1985-01-01

    The production of radionuclides for medical and biomedical research in Canada has been reviewed with respect to the national geographic and demographic characteristics which influence their use. The types of facilities available for the production of short-lived radionuclides have been summarized, and a tabulation of the radionuclides that are produced has been presented. In broad terms production facilities can be classified as belonging to one of two groups, nuclear reactor or charged-particle accelerators. The charged-particle accelerators produce the more neutron-deficient and (because of the resultant decay properties) the more useful radionuclides for medical application. The nuclear reactor facilities for radionuclide production range in size and capacity from the high-flux research reactors of AECL to the six SLOWPOKE reactors, five of which are located on university campuses across the country. The McMaster University reactor is used to produce curie quantities of fluorine-18 weekly. Millicurie amounts of a large number of radionuclides, most of which have half-lives ranging from 2 to 50 hr, are produced in the low-flux reactors, in support of basic medical research

  4. Feasibility of short-lived radionuclide production at Fermilab

    International Nuclear Information System (INIS)

    Ten Haken, R.K.; Awschalom, M.; Rosenberg, I.

    1985-01-01

    The requirements for establishing a short-lived radionuclide production program at Fermilab are explored. Such a program would utilize beam from the linac portion of the injector much like the present Neutron Therapy Facility. It should be possible to use approximately 10 to 20 μA of 66-MeV protons for iodine-123 production. Several additional magnets would need to be acquired and a shielded target facility would need to be constructed. However, the feasibility of establishing such a program hinges upon its harmonious operation with the high energy physics program

  5. Kinetic aspects of the syntheses using short-lived radionuclides

    International Nuclear Information System (INIS)

    Laangstroem, B.; Obenius, U.; Sjoeberg, S.; Bergson, G.

    1981-01-01

    In syntheses using short-lived radionuclides, such as 11 C, the reaction conditions are usually such that the concentrations of the reactants, except for the labelled reactant, can be considered constant during the reaction. Two kinetic models have been investigated - irreversible and reversible bimolecular elementary reactions. The influence of the rate constants, of the equilibrium constants, and of the ratio between the starting reactants on the yield of the labelled product has been studied. The results show that, even in cases with unfavourable equilibrium constants, high yields of the labelled products can be obtained if the rate constant for the forward reaction is large. In addition, the specific activity of the labelled product as a function of time has been studied for the irreversible bimolecular case. (author)

  6. Fast neutron activation analysis using short-lived radionuclides

    International Nuclear Information System (INIS)

    Salma, I.; Zemplen-Papp, E.

    1993-01-01

    Fast neutron activation analysis experiments were performed to investigate the analytical possibilities and prospective utilization of short-lived activation products. A rapid pneumatic transfer system for use with neutron generators has been installed and applied for detecting radionuclides with a half-life from ∼300 ms to 20 s. The transport time for samples of total mass of 1-4 g is between 130 and 160 ms for pressurized air of 0.1-0.4 MPa. The reproducibility of transport times is less than 2%. The employed method of correcting time-dependent counting losses is based on the virtual pulse generator principle. The measuring equipment consists of CAMAC modules and a special gating circuit. Typical time distributions of counting losses are presented. The same 14 elements were studied by the conventional activation method (single irradiation and single counting) by both a typical pneumatic transport system (run time 3 s) and the fast pneumatic transport facility. Furthermore, the influence of the cyclic activation technique on the elemental sensitivities was investigated. (author) 15 refs.; 5 figs.; 3 tabs

  7. Interest of the Department of Energy in production and development of short-lived radionuclides

    International Nuclear Information System (INIS)

    Thiessen, J.W.

    1985-01-01

    The Department of Energy has developed production of potentially useful radionuclides for applications in medicine. The Department's financial commitment and the short-lived radionuclide production program, with emphasis on iodine-123, is discussed

  8. Developing role of short-lived radionuclides in nuclear medical practice. DOE symposium series; 56

    International Nuclear Information System (INIS)

    Paras, P.; Thiessen, J.W.

    1985-01-01

    The purpose was to define the developing role and state-of-the-art development of short-lived radionuclides (SLR's) in current nuclear medical practice. Special emphasis was placed on radionuclides with general-purpose labeling capabilities. The need for high-purity labeling-grade iodine-123 was emphasized in the program. Papers have been separately abstracted for the data base

  9. History and review of short-lived radionuclide development

    International Nuclear Information System (INIS)

    Myers, W.G.

    1985-01-01

    The use of twinkling atoms in biomedicine is discussed from the historical point of view. Their discovery, production, and applications are described. The development of modern nuclear medicine from its inception, e.g., the first simple applications, to the latest complex studies are described with special emphasis on the applications of the ideal radionuclide - iodine-123

  10. Application of accelerator-produced short-lived radionuclides in industry

    International Nuclear Information System (INIS)

    Kupsch, H.

    1986-01-01

    Several problems such as corrosion, catalysis, wear, process optimization and diagnosis, damage analysis, arising in idustry can be solved using short-lived radioisotopes. Some examples of technological target designs which have been developed are demonstrated for the radionuclide production based on p,n; d,α; α,n; α,2n; α,p; γ,n; γ,p nuclear reactions. Applications of short-lived radionuclides in plants and processes of electrodeposition and gas concrete production are described. (author)

  11. Synthesis of radiopharmaceuticals containing short-lived radionuclides. Comprehensive report, March 1, 1980-February 26, 1986

    International Nuclear Information System (INIS)

    Kabalka, G.W.

    1985-09-01

    New methods for the rapid introduction of short-lived radionuclides into agents for use in diagnostic nuclear medicine are reported. Among the new syntheses reported are those for 123 I-labeled fatty acids and steroids, for 11 C-labeled alcohols, for 13 N-labeled amines, and for 15 O-labeled alcohols. 33 refs

  12. Synthesis of radiopharmaceuticals containing short-lived radionuclides. Progress report, March 1, 1985-February 26, 1986

    International Nuclear Information System (INIS)

    Kabalka, G.W.

    1985-09-01

    Methods for the rapid introduction of short-lived radionuclides into agents for use in diagnostic nuclear medicine are reported. Methods to synthesize radioiodinated fatty acids, lipids, and amphetamine derivatives are described. New routes for the introduction of bromine-77, chlorine-34m, and carbon-11 into agents of interest are elaborated. 46 refs

  13. Development of the k0-based cyclic neutron activation analysis for short-lived radionuclides

    NARCIS (Netherlands)

    Dung, H.M.; Blaauw, M.; Beasley, D.; Freitas, M.D.C.

    2011-01-01

    The k0-based cyclic neutron activation analysis (k0-CNAA) technique has been studied to explore the applicability at the Portuguese research reactor (RPI). In particular, for the determination of elements which form short-lived radionuclides, particularly fluorine (20F, 11.16 s half-life) and

  14. Review of short-lived radionuclide activities in the United States

    International Nuclear Information System (INIS)

    Sodd, V.J.

    1985-01-01

    A review is given of the accelerator-produced short-lived radionuclides which are used in radiopharmaceuticals available commercially in the US and of the accelerator facilities devoted primarily to their production. Reactions for the efficient production of 67 Ga, 81 Rb → /sup 81m/Kr, 111 In, 201 Tl, and 123 I are given. Methods for the production of higher purity 123 I are suggested

  15. Short-lived radionuclide production capability at the Brookhaven Linac Isotope Producer

    International Nuclear Information System (INIS)

    Mausner, L.F.; Richards, P.

    1985-01-01

    The Brookhaven National Linac Isotope Producer is the first facility to demonstrate the capability of a large linear accelerator for efficient and economical production of difficult-to-make, medically useful radionuclides. The linac provides a beam of 200-MeV protons at an integrated beam current of up to 60 μA. The 200-MeV proton energy is very suitable for isotope production because the spallation process can create radionuclides unavailable at lower energy accelerators or reactors. Several medically important short-lived radionuclides are presently being prepared for on-site and off-site collaborative research programs. These are iodine-123, iron-52, manganese-52m, ruthenium-97, and the rubidium-81-krypton-81m system. The production parameters for these are summarized

  16. Non-destructive investigation of technical plants and processes and natural processes by short-lived radionuclides (radiotracer)

    International Nuclear Information System (INIS)

    Jentsch, Thorsten; Zeuner, Albert

    2009-01-01

    Short lived open radionuclides are very suitable to investigate transport and mixing processes. They do not pollute the product. After decay of the radionuclide, the product can be used without any restrictions. Examples are showed for technical processes investigation by aid of radiotracer. (orig.)

  17. External tandem target system for efficient production of short-lived positron emitting radionuclides

    International Nuclear Information System (INIS)

    Koh, K.; Dwyer, J.; Finn, R.; Sheh, Y.; Sinnreich, J.; Wooten, T.

    1983-01-01

    Recent developments in radiopharmaceutical chemistry allow the incorporation of short-lived, positron-emitting radionuclides into a variety of compounds which when used with a positron emission tomograph provide a means of monitoring physiological disorders by a standard technique. To effectively meet the increased ''in-house'' clinical demands while maintaining a production schedule, a tandem target was designed and has been installed for the simultaneous ''on-line'' preparation of oxygen-15 labelled compounds such as CO 2 15 , H 2 O 15 ; and nitrogen-13 labelled compounds such as 13 NH 3 , 13 N 2 O, and 13 N 2 . The processing time required for the synthesis of the nitrogen-13 products as compared to the essentially instantaneous formation of oxygen-15 labelled compounds has provided the necessary time delay for clinical utilization. The characterisitcs of this external tandem target system as well as the automation for the dual processing are presented

  18. Monitoring of processes with gamma-rays of neutron capture and short-living radionuclides

    International Nuclear Information System (INIS)

    Aripov, G.A.; Kurbanov, B.I.; Allamuratova, G.

    2004-01-01

    Element content is a fundamental parameter of a substance, on which all its properties, and also character of physical, chemical, biological, technological and ecological processes depend. Therefore monitoring of element content (in the course of technological process - on line; in natural conditions - in site; or in living organisms - in vivo) becomes necessary for investigation of aforementioned processes. This problem can be successfully solved by using the methods of prompt gamma activation analysis (PGAA) and instrumental neutron activation analysis (INAA) on short-living radionuclides. These methods don't depend on type of substance (biological, geological, technological etc.), since the content is determined by gamma radiation of nuclei, and allows to meet such a serious requirement like the necessity of achieving minimal irradiation of the object and its minimal residual activity. In this work minimal determinable concentrations of various elements are estimated (based on experimental data) by the method of PGAA using radionuclide 252 Cf - source of neutrons with the yield of the oil of 10 8 neutron/sec on the experimental device with preliminary focusing of neutrons /1/, and also data of determination of elements by their isotopes with maximum time efficiency /2,3/ by the method of INAA. (author)

  19. Labeling suspended aerosol particles with short-lived radionuclides for determination of particle deposition

    International Nuclear Information System (INIS)

    Smith, M.F.; Bryant, S.; Welch, S.; Digenis, G.A.

    1984-01-01

    Radiotracer techniques were developed to examine parameters that characterize pressurized aerosols designed to deliver insoluble particles suspended in the aerosol formulation. Microaggregated bovine serum albumin microspheres that were to be suspended were labeled with iodine-131 (t1/2 . 8 d). This iodination procedure (greater than 80% effective) is also applicable to iodine-123, which possesses superior characteristics for external imaging and further in vivo studies. This report shows that for pressurized aerosols containing suspended particles, each metered dose is approximately equal (not including the priming doses and the emptying doses). Increase in the delivery of the albumin particles out of the canister was best achieved by pretreating the valve assembly with a solution of 2% (w/v) bovine serum albumin in phosphate buffer. Use of a cascade impactor delineated the particle size distribution of the micropheres, with the majority of particles ranging in size from 2 to 8 microns. The data disclosed here indicate that the techniques developed with short-lived radionuclides can be used to quantitate each metered dose, characterize the particle size distribution profile of the aerosol contents, and determine the extent of deposition of the particles in the aerosol canister and all of its components

  20. Sediment-associated transport and redistribution of Chernobyl fallout radionuclides

    International Nuclear Information System (INIS)

    Walling, D.E.; Rowan, J.S.; Bradley, S.B.

    1989-01-01

    Fallout of Chernobyl-derived radionuclides over the United Kingdom evidenced marked spatial variation. Relatively high levels were recorded in central Wales, but they declined rapidly to the east. As a result the headwaters of the River Severn received significant inputs of fallout, whereas only low levels were recorded over the middle and lower reaches. Measurements of the caesium-137 content of suspended sediment transported by the River Severn and of channel and floodplain sediments collected from various locations within the basin have been used to assess the importance of fluvial transport and redistribution of Chernobyl-derived radionuclides. High concentrations of caesium-137 (up to 1450 mBqg -1 ) were recorded in suspended sediment collected from the lower reaches of the river shortly after the Chernobyl incident and substantial accumulations of Chernobyl-derived radionuclides have been detected in floodplain and channel sediments collected from areas which received only low levels of fallout directly. (author)

  1. Vertical soil migration of radionuclide fallout from the Chernobyl' accident

    International Nuclear Information System (INIS)

    Silant'ev, A.N.; Shkuratova, I.G.; Bobovnikova, T.I.

    1989-01-01

    The most suitable model for describing the behavior of radionuclide fallout on a soil surface is quasidiffusion transfer with directional transfer taken into account. The parameter values for this have been determined previously and are supplemented by the results of this work. To investigate the initial radionuclide distribution along the soil profile, monolithic soil samples 5 cm thick were taken in June-September 1986 in areas which had been subjected to contamination due to the Chernobyl' accident. The samples taken were cut up into layers. The first layer, 0.5 cm thick, was cut off from the surface of the soil monolith together with the grass. The next layer cut off was also 0.5 cm thick. Then two layers, each 1 cm in thickness, were cut off. The thickness of the last layer was 2 cm. The vertical distribution of radionuclides along the soil profile which was examined may be called the initial distribution, which will then change due to nonimmediate migration of radionuclides in the soil. Based on the research which has been performed, the following conclusions may be drawn. One portion of the radionuclides resulting from fallout is trapped by plant cover, while the other enters immediately into the soil. For a thick plant covering, about 80% of the radionuclide fallout is sorbed by the grass; for sparse cover, about 40%. The radionuclides entering the soil along with rainwater penetrate into the soil depths, producing contamination which falls off exponentially with depth. The exponent index is close to 1 cm -1 . In a forest, the main amount of radionuclide fallout is trapped by litter. Approximately 10% of the contamination fallout penetrates beneath the litter

  2. Production cross sections of short-lived silver radionuclides from natPd(p,xn) nuclear processes

    International Nuclear Information System (INIS)

    Khandaker, Mayeen Uddin; Kim, Kwangsoo; Kim, Guinyun

    2012-01-01

    Production cross-sections of short-lived 103 Ag, 104m Ag and 104g Ag radionuclides from proton-induced reactions on natural palladium (Pd) were measured up to 41 MeV by using a stacked-foil activation technique combined with high resolution γ-ray spectrometry. The present results are compared with the available literature values as well as theoretical data calculated by the TALYS and the ALICE-IPPE computer codes. Note that production cross-sections of the 104m Ag radionuclide from nat Pd(p,xn) processes has been measured here for the first time. Physical thick target yields for the investigated radionuclides were deduced from the respective threshold energy to 41 MeV taking into account that the total energy is absorbed in the targets. Measured data of the short-lived 103 Ag radionuclide are noteworthy due to its possible applications as a precursor for the indirect production of widely used therapeutic 103 Pd radionuclide via nat Pd(p,xn) 103 Ag → 103 Pd processes. On the other hand, the investigated 104 Ag radionuclide finds importance due to its potential use as a diagnostic and positron emission tomography (PET) imaging analogue. Above all, measured data will enrich the literature database leading to various applications in science and technology.

  3. Content of short-lived radionuclides in the Kanevskoe water reservoir and its coastal ecosystems after the Chernobyl NPP accident

    International Nuclear Information System (INIS)

    Zarubin, O.L.

    2008-01-01

    The content of Te 132, Np 239, Ba 140, I 131 in components of ecosystem of Kanevskoe reservoir of river Dnepr and adjoining to it surface ecosystems studied in 1986. The maximal content of investigated radionuclides was registered in water and surface vegetation. Contamination of hydrobionts by Ba 140 and I 131 has been generated practically at once after fall-out of these radionuclides directly on a mirror of the reservoir during the period from 30.04.1986 to 02.05.1986. Cancers Astacus Leptodactilus Eichw. and fishes intensively accumulated Ba 140 and I 131. (authors)

  4. Use of short-lived radionuclides in the agricultural and environmental sciences

    International Nuclear Information System (INIS)

    Krohn, K.A.

    1985-01-01

    In addition to their well-known uses in physiology, biochemistry, and medicine, short-lived radioisotopes have played an important part in promoting the authors knowledge of the agricultural and environmental sciences. Numerous investigators have found that the scientific rewards justify the additional demands associated with use of short-lived radioisotopes when novel or uniquely precise results can be achieved. This is best exemplified by examining the use of 13 N. Nitrogen-13 is the longest lived radioisotope of this very important element. The 10-min half-life of 13 N has required that the agricultural or environmental test model be brought to the laboratory where the isotope is made, but this has been done successfully in numerous instances. One major incentive for this research has probably been the fact that there is no analog of the very useful 14 C tracer to study nitrogen chemistry and biology

  5. Behaviour of Chernobyl fallout radionuclides deposited on peat and urban surfaces in Finland

    International Nuclear Information System (INIS)

    Reponen, A.

    1992-10-01

    In the thesis the impact of the Chernobyl nuclear reactor accident on Finland was studied in three aspects: (1) the areal distribution of Chernobyl fallout in Finland was determined by measuring peat samples, (2) the behaviour of fallout radionuclides was investigated in the combustion of peat in power plants, and (3) the removal rates of fallout radionuclides on urban surfaces were resolved

  6. Global deposition of fallout radionuclides and their dietary intake

    International Nuclear Information System (INIS)

    Morisawa, Shinsuke

    1993-01-01

    Japanese foods depend largely on foreign countries and domestic food supply now is no more than 30 percents if feedstuffs for live-stocks are included. Therefore not only ecological/natural but also social, e.g., human activities related, transportation of fallout radionuclides are to be taken into accounts for estimation of baseline internal irradiation dose and health risks of Japanese peoples through dietary intake of radionuclides. In this study, mathematical model is developed and examined for practical application on estimating Japanese dietary intake level of fallout strontium-90, which is accumulated in various kinds of foodstuffs and is transported to Japan associated with worldwide trades of foods, under appropriate limitations such that direct deposition on plants and seafood intake pathways are not evaluated. Deposition of strontium-90 onto the surface soil was simulated using the model, the compartment model described by a set ordinary differential equations, and the estimates were examined by comparing them with the observed data colleted and complied by the global scale environmental monitoring networks. Sensitivity analysis is also practised to find possible reduction of dietary intake of fallout radionuclides and the related potential health risks. (author)

  7. Corrections for the combined effects of decay and dead time in live-timed counting of short-lived radionuclides

    International Nuclear Information System (INIS)

    Fitzgerald, R.

    2016-01-01

    Studies and calibrations of short-lived radionuclides, for example "1"5O, are of particular interest in nuclear medicine. Yet counting experiments on such species are vulnerable to an error due to the combined effect of decay and dead time. Separate decay corrections and dead-time corrections do not account for this issue. Usually counting data are decay-corrected to the start time of the count period, or else instead of correcting the count rate, the mid-time of the measurement is used as the reference time. Correction factors are derived for both those methods, considering both extending and non-extending dead time. Series approximations are derived here and the accuracy of those approximations are discussed. - Highlights: • Derived combined effects of decay and dead time. • Derived for counting systems with extending or non-extending dead times. • Derived series expansions for both midpoint and decay-to-start-time methods. • Useful for counting experiments with short-lived radionuclides. • Examples given for "1"5O, used in PET scanning.

  8. Synthesis of radiopharmaceuticals containing short-lived radionuclides: Progress report, March 1, 1987-February 28, 1988

    International Nuclear Information System (INIS)

    Kabalka, G.W.

    1987-09-01

    The objective is the creation of new methods for introducing short-lived isotopes into agents for use in diagnostic nuclear medicine. Focus is on the design of new molecular architecture as opposed to the application of known reactions to the synthesis of specific radiopharmaceuticals. The new technology is utilized in nuclear medicine research at the University of Tennessee Medical Imaging Center and in collaboration with colleagues at other DOE facilities. The program provides training for students in the scientific aspects of nuclear medicine. The academic nature of the program facilitates collaborative interactions with other DOE nuclear medicine programs and helps to insure the continued availability of skilled scientists dedicated to the advancement of nuclear medicine. 70 refs., 9 figs

  9. Sorption of short-lived radionuclides in a layer of sorbent with spherical granules

    International Nuclear Information System (INIS)

    Karlin, Yu.V.

    1993-01-01

    Sorption methods have found wide application in the purification of liquid radioactive wastes. The working element in sorption methods for this purpose is usually a sorption column with a fixed layer of sorbent. Continuous-action equipment with a moving layer of sorbent is very seldom used. When a fixed layer of sorbent is used its wear and prolonged mixing in the sorption column are reduced to a minimum, and maximum purification is achieved due to the advantages of the dynamic method of sorption over the static method. The time of protective action of the sorbent layer is determined by the time taken for the radionuclide to pass through the sorption column, and for the majority of radionuclides is determined by numerous parameters, including the type of sorbent and radionuclide, the rate of flow through the sorbent, the size of the sorbent granules, etc. The physical and chemical aspects of this process have been investigated in detail, and numerous methods for modeling it mathematically have been developed and have been used to develop methods of designing sorption column apparatus. The specific nature of the radionuclides as unstable materials enables the hypothetical case of a open-quotes perpetualclose quotes sorption filter to be represented. In fact, to achieve this it is only necessary to assume that the half-life of the radionuclide is so small that the rate of decay of the radionuclide in the sorption column (both in the sorbed state and in the aqueous phase of the sorption layer) is equal to the rate that it is fed into the column in the flow of liquid radioactive waste. In this case the sorption front of the radionuclide in the column wall remains fixed after a certain initial period. In this paper, a mathematical model of such a hypothetical filter for the case of spherical sorbent granules is considered

  10. Short-lived radionuclides produced on the ORNL 86-inch cyclotron and High-Flux Isotope Reactor

    International Nuclear Information System (INIS)

    Lamb, E.

    1985-01-01

    The production of short-lived radionuclides at ORNL includes the preparation of target materials, irradiation on the 86-in. cyclotron and in the High Flux Isotope Reactor (HFIR), and chemical processing to recover and purify the product radionuclides. In some cases the target materials are highly enriched stable isotopes separated on the ORNL calutrons. High-purity 123 I has been produced on the 86-in. cyclotron by irradiating an enriched target of 123 Te in a proton beam. Research on calutron separations has led to a 123 Te product with lower concentrations of 124 Te and 126 Te and, consequently to lower concentrations of the unwanted radionuclides, 124 I and 126 I, in the 123 I product. The 86-in. cyclotron accelerates a beam of protons only but is unique in providing the highest available beam current of 1500 μA at 21 MeV. This beam current produces relatively large quantities of radionuclides such as 123 I and 67 Ga

  11. Harvard--MIT research program in short-lived radiopharmaceuticals. Progress report, September 1, 1977--April 30, 1978. [/sup 99m/Tc, positron-emitting radionuclides

    Energy Technology Data Exchange (ETDEWEB)

    Adelstein, S.J.; Brownell, G.L.

    1978-05-01

    Progress is reported on the following studies: chemistry studies designed to achieve a more complete understanding of the fundamental chemistry of technetium in order to facilitate the design of future radiopharmaceuticals incorporating the radionuclide /sup 99m/Tc; the development of new radiopharmaceuticals intended to improve image quality and lower radiation doses by the use of short-lived radionuclides and disease-specific agents; the development of short-lived positron-emitting radionuclides which offer advantages in transverse section imaging of regional physiological processes; and studies of the toxic effects of particulate radiation.

  12. The utilisation of short-lived radionuclides in the assessment of formulation and in vivo disposition of drugs

    International Nuclear Information System (INIS)

    Digenis, G.A.

    1982-01-01

    The utilisation of short-lived radionuclides in the assessment of drug formulations, and the in vivo distribution of drugs is discussed. Disintegration of tablets and capsules as a function of the formulation, and gastric emptying are important. The applicability of perturbed angular correlation to the study of the dissolution of water soluble substances from solid dosages in man is shown. Examples are given to illustrate how external scintigraphy can be applied to study the tissue distribution of 18 F-haloperidol, 82 Br-bromperidol, in rat and monkey. 11 C, L-andD-phenylalanine in rats, 11 C, D-leucine in mice with human colon tumours; 13 N-nitrosoureas and 13 N-nitroso-carbamates. (U.K.)

  13. Contribution of the short lived radionuclides in food to the total radiation burden of man after the nuclear accident in Chernobyl

    International Nuclear Information System (INIS)

    Popovic, D.; Djuric, G.; Smelcerovic, M.; Maksimovic, B.

    1989-01-01

    The paper presents the results of the short lived radionuclides (I-131, Te(I)-132, Cs-136, Ce-141,144, Ru-103,106, Ba(La)-140, Zr-95, Mo-99, Nb-95, Sb-125) mass activities estimation in some foodstuff (milk and milk products), immediately after the nuclear accident in Chernobyl, in May 1986. The activities of the radionuclides were determined on Ge(Li) detector by standard gamma spectrometry, with the total error less than 20%. The results enabled the evaluation of the short lived radionuclides contribution in the total dose due to ingestion of milk and milk products, in the first month after the accident, compared to the contribution of I-131 and to the contribution of the main long lived radionuclides: Ce-134 and Cs-137 (author)

  14. Redistribution of fallout radionuclides in Enewetak Atoll lagoon sediments by callianassid bioturbation

    Energy Technology Data Exchange (ETDEWEB)

    McMurtry, G.M.; Schneider, R.C. (Hawaii Univ., Honolulu (USA). Hawaii Inst. of Geophysics); Colin, P.L. (Hawaii Inst. of Marine Biology, Honolulu (USA)); Buddemeier, R.W. (California Univ., Livermore (USA). Lawrence Livermore Lab.); Suchanek, T.H. (Fairleigh Dickinson Univ., St. Croix, Virgin Islands (USA). West Indies Lab.)

    1985-02-21

    The lagoon sediments of Enewetak Atoll in the Marshall Islands contain a large selection of fallout radionuclides as a result of 43 nuclear weapon tests conducted there between 1948 and 1958. The authors report elevated fallout radionuclide concentrations buried more deeply in the lagoon sediments and evidence of burrowing into the sediment by several species of callianassid ghost shrimp (Crustacea: Thalassinidea) which has displaced highly radioactive sediment. The burrowing activities of callianassids, which are ubiquitous on the lagoon floor, facilitate radionuclide redistribution and complicate the fallout radionuclide inventory of the lagoon.

  15. Redistribution of fallout radionuclides in Enewetak Atoll lagoon sediments by callianassid bioturbation

    International Nuclear Information System (INIS)

    McMurtry, G.M.; Schneider, R.C.; Buddemeier, R.W.; Suchanek, T.H.

    1985-01-01

    The lagoon sediments of Enewetak Atoll in the Marshall Islands contain a large selection of fallout radionuclides as a result of 43 nuclear weapon tests conducted there between 1948 and 1958. The authors report elevated fallout radionuclide concentrations buried more deeply in the lagoon sediments and evidence of burrowing into the sediment by several species of callianassid ghost shrimp (Crustacea: Thalassinidea) which has displaced highly radioactive sediment. The burrowing activities of callianassids, which are ubiquitous on the lagoon floor, facilitate radionuclide redistribution and complicate the fallout radionuclide inventory of the lagoon. (author)

  16. Redistribution of fallout radionuclides in Enewetak Atoll lagoon sediments by callianassid bioturbation.

    Science.gov (United States)

    McMurtry, G M; Schneider, R C; Colin, P L; Buddemeier, R W; Suchanek, T H

    The lagoon sediments of Enewetak Atoll in the Marshall Islands contain a large selection of fallout radionuclides as a result of 43 nuclear weapon tests conducted there between 1948 and 1958. Studies of the burial of fallout radionuclides have been conducted on the islands and in several of the large craters, but studies of their vertical distribution have been limited to about the upper 20 cm of the lagoon sediments. We have found elevated fallout radionuclide concentrations buried more deeply in the lagoon sediments and evidence of burrowing into the sediment by several species of callianassid ghost shrimp (Crustacea: Thalassinidea) which has displaced highly radioactive sediment. The burrowing activities of callianassids, which are ubiquitous on the lagoon floor, facilitate radionuclide redistribution and complicate the fallout radionuclide inventory of the lagoon.

  17. The effects of short-lived radionuclides and porosity on the early thermo-mechanical evolution of planetesimals

    Science.gov (United States)

    Lichtenberg, Tim; Golabek, Gregor J.; Gerya, Taras V.; Meyer, Michael R.

    2016-08-01

    The thermal history and internal structure of chondritic planetesimals, assembled before the giant impact phase of chaotic growth, potentially yield important implications for the final composition and evolution of terrestrial planets. These parameters critically depend on the internal balance of heating versus cooling, which is mostly determined by the presence of short-lived radionuclides (SLRs), such as 26Al and 60Fe, as well as the heat conductivity of the material. The heating by SLRs depends on their initial abundances, the formation time of the planetesimal and its size. It has been argued that the cooling history is determined by the porosity of the granular material, which undergoes dramatic changes via compaction processes and tends to decrease with time. In this study we assess the influence of these parameters on the thermo-mechanical evolution of young planetesimals with both 2D and 3D simulations. Using the code family I2ELVIS/I3ELVIS we have run numerous 2D and 3D numerical finite-difference fluid dynamic models with varying planetesimal radius, formation time and initial porosity. Our results indicate that powdery materials lowered the threshold for melting and convection in planetesimals, depending on the amount of SLRs present. A subset of planetesimals retained a powdery surface layer which lowered the thermal conductivity and hindered cooling. The effect of initial porosity was small, however, compared to those of planetesimal size and formation time, which dominated the thermo-mechanical evolution and were the primary factors for the onset of melting and differentiation. We comment on the implications of this work concerning the structure and evolution of these planetesimals, as well as their behavior as possible building blocks of terrestrial planets.

  18. IN-SITU RADIONUCLIDE TRANSPORT NEAR THE NOPAL I URANIUM DEPOSIT AT PENA BLANCA, MEXICO: CONSTRAINTS FROM SHORT-LIVED DECAY-SERIES RADIONUCLIDES

    International Nuclear Information System (INIS)

    Luo, S.; Ku, T.L.; Todd, V.; Murrell, M.; Pineda, J. Alfredo Rodriguez; Dinsmoor, J.; Mitchell, A.

    2005-01-01

    For nuclear waste management, an important mechanism by which radioactive waste components are isolated from returning to the human environment, the biosphere, is by the geological barrier in which the effectiveness of the barrier is characterized by in-situ retardation factor, i.e., the transport rate of a radionuclide relative to that of groundwater. As part of natural analog studies of the Yucca Mountain Project of the U. S. Department of Energy, we propose such characterization by using naturally-occurring decay-series radioisotopes as an analog. We collected large-volume (>1000 liters) groundwater samples from three wells (PB, Pozos, and PB4, respectively) near the Nopal I Uranium Ore site at Pena Blanca, Mexico, by using an in-situ Mn-cartridge filtration technique for analysis of short-lived decay-series radionuclides. Results show that the activities of short-lived radioisotopes ( 228 Ra, 224 Ra and 223 Ra) and activity ratios of 224 Ra/ 228 Ra and 224 Ra/ 223 Ra are higher at PB and Pozos than at PB4. In contrast, the 210 Po activity is much lower at PB and Pozos than at PB4. The high Ra activities and activities ratios at PB and Pozos are attributable to the high alpha-recoil input from the aquifer rocks, while the high 210 Po activity at PB4 is due to the enhanced colloidal transport. Based on a uranium-series transport model, we estimate that the in-situ retardation factor of Ra is (0.43 ± 0.02) x 10 3 at PB, (1.68 ± 0.08) x 10 3 at Pozos, and (1.19 ± 0.08) x 10 3 at PB4 and that the mean fracture width in the aquifer rocks is about 0.23 (micro)m at PB, 0.37 (micro)m at Posos, and 4.0 (micro)m at PB4, respectively. The large fracture width at PB4 as derived from the model provides an additional evidence to the inference from the Po measurements that particle-reactive radionuclides are transported mainly as colloidal forms through the large fractures in rocks. Our model also suggests that in addition to alpha recoil, decay of 226 Ra from the adsorbed

  19. IN-SITU RADIONUCLIDE TRANSPORT NEAR THE NOPAL I URANIUM DEPOSIT AT PENA BLANCA, MEXICO: CONSTRAINTS FROM SHORT-LIVED DECAY-SERIES RADIONUCLIDES

    Energy Technology Data Exchange (ETDEWEB)

    S. Luo; T.L. Ku; V. Todd; M. Murrell; J. Alfredo Rodriguez Pineda; J. Dinsmoor; A. Mitchell

    2005-07-11

    For nuclear waste management, an important mechanism by which radioactive waste components are isolated from returning to the human environment, the biosphere, is by the geological barrier in which the effectiveness of the barrier is characterized by in-situ retardation factor, i.e., the transport rate of a radionuclide relative to that of groundwater. As part of natural analog studies of the Yucca Mountain Project of the U. S. Department of Energy, we propose such characterization by using naturally-occurring decay-series radioisotopes as an analog. We collected large-volume (>1000 liters) groundwater samples from three wells (PB, Pozos, and PB4, respectively) near the Nopal I Uranium Ore site at Pena Blanca, Mexico, by using an in-situ Mn-cartridge filtration technique for analysis of short-lived decay-series radionuclides. Results show that the activities of short-lived radioisotopes ({sup 228}Ra, {sup 224}Ra and {sup 223}Ra) and activity ratios of {sup 224}Ra/{sup 228}Ra and {sup 224}Ra/{sup 223}Ra are higher at PB and Pozos than at PB4. In contrast, the {sup 210}Po activity is much lower at PB and Pozos than at PB4. The high Ra activities and activities ratios at PB and Pozos are attributable to the high alpha-recoil input from the aquifer rocks, while the high {sup 210}Po activity at PB4 is due to the enhanced colloidal transport. Based on a uranium-series transport model, we estimate that the in-situ retardation factor of Ra is (0.43 {+-} 0.02) x 10{sup 3} at PB, (1.68 {+-} 0.08) x 10{sup 3} at Pozos, and (1.19 {+-} 0.08) x 10{sup 3} at PB4 and that the mean fracture width in the aquifer rocks is about 0.23 {micro}m at PB, 0.37 {micro}m at Posos, and 4.0 {micro}m at PB4, respectively. The large fracture width at PB4 as derived from the model provides an additional evidence to the inference from the Po measurements that particle-reactive radionuclides are transported mainly as colloidal forms through the large fractures in rocks. Our model also suggests that

  20. Fallout Radionuclides as Tracers in Southern Alps Sediment Studies

    Science.gov (United States)

    Carey, A. E.; Karanovic, Z.; Dibb, J. E.

    2005-12-01

    The primary geologic processes shaping the landscape are physical and chemical weathering and the transport of solids by erosion. As part of our studies on the coupling between physical erosion and chemical weathering, we have determined depositional and erosional processes in New Zealand's tectonically active, rapidly uplifting Southern Alps, specifically focusing on the Hokitika River watershed. The South Island watersheds we are studying are subject to extreme orographic precipitation (as high as 7-12 m annually) and high landslide frequency, but have modest topography due to the rapid erosion. In concert with our studies of chemical weathering and physical erosion, we have used the atmospherically-delivered radionuclides of 7Be, 137Cs and 210Pbexcess to determine the relative magnitude of particle residence time in the high elevation Cropp and Whitcombe subwatersheds and the rates of sedimentation. One- and two-box modeling with 7Be and 210Pbexcess was used to determine soil and sediment residence times. Residence time of fine suspended particles is short and particles can travel the length of the river during a single storm, probably due to the short duration, high-intensity rainfalls which produce rapidly moving, steep flood waves. The readily detected peak of 137Cs activity in Cropp terrace and Hokitika gorge soils yielded sedimentation rates of 0.06-0.12 cm yr-1. At the Cropp terrace, inventory models of 210Pbexcess yield soil accumulation rates significantly less than those determined using the 137Cs activity peak. We attribute the differences to overestimation of 210Pbexcess in surface soils and to contrasting fallout fluxes, geochemical behavior and radionuclide contents of sedimenting materials. Total inventories of 210Pbexcess in soils greatly exceed the expected direct atmospheric deposition, suggesting that lateral transport of this nuclide occurs within the watershed. At the Hokitika gorge, all nuclides studied yielded similar sedimentation rates

  1. Overview of past activities for the use of short-lived radionuclides and the role of the Bureau of Radiological Health

    International Nuclear Information System (INIS)

    Paras, P.

    1985-01-01

    The Bureau of Radiological Health has developed a national program to control unnecessary medical radiation exposures to man and to assure the safe and effective use of radiation. The continuing interest and the role of the Bureau in the use of short-lived radionuclides (SLR's) are emphasized. An overview of the Bureau's SLR program, past accomplishments, and the status of production and use of iodine-123 are presented

  2. Estimated inventory of plutonium and uranium radionuclides for vegetation in aged fallout areas

    International Nuclear Information System (INIS)

    Romney, E.M.; Wallace, A.; Kinnear, J.; Gilbert, R.O.

    1977-01-01

    Data are presented pertinent to the contamination of vegetation by plutonium and other radionuclides in aged fallout areas on the Nevada Test Site (NTS) and the Tonopah Test Range (TTR). The standing biomass of vegetation estimated by nondestructive dimensional methods varied from about 200 to 600 g/m 2 for the different fallout areas. Estimated inventories of 238 Pu, 239 Pu, 240 Pu, and 235 U in plants and their biological effects are discussed

  3. A general dead-time correction method based on live-time stamping. Application to the measurement of short-lived radionuclides.

    Science.gov (United States)

    Chauvenet, B; Bobin, C; Bouchard, J

    2017-12-01

    Dead-time correction formulae are established in the general case of superimposed non-homogeneous Poisson processes. Based on the same principles as conventional live-timed counting, this method exploits the additional information made available using digital signal processing systems, and especially the possibility to store the time stamps of live-time intervals. No approximation needs to be made to obtain those formulae. Estimates of the variances of corrected rates are also presented. This method is applied to the activity measurement of short-lived radionuclides. Copyright © 2017 Elsevier Ltd. All rights reserved.

  4. Ground depositions and air concentrations of Chernobyl fallout radionuclides at Munich-Neuherberg

    Energy Technology Data Exchange (ETDEWEB)

    Hoetzl, H.; Rosner, G.; Winkler, R.

    1987-01-01

    Southern Bavaria has received a comparatively high deposition of fallout radionuclides from the reactor accident at Chernobyl. As a result, in addition to the measurement of numerous gamma emitting nuclides and of strontium isotopes, the determination of several actinides, including isotopes of uranium, neptunium, plutonium and curium was possible. The observed radionuclide composition of the fallout and the time course of ground deposition and air concentration at the site of the Gesellschaft fuer Strahlen- und Umweltforschung (GSF) at Neuherberg, 10 km north of Munich, are reported and discussed.

  5. Ground depositions and air concentrations of Chernobyl fallout radionuclides at Munich-Neuherberg

    International Nuclear Information System (INIS)

    Hoetzl, H.; Rosner, G.; Winkler, R.

    1987-01-01

    Southern Bavaria has received a comparatively high deposition of fallout radionuclides from the reactor accident at Chernobyl. As a result, in addition to the measurement of numerous gamma emitting nuclides and of strontium isotopes, the determination of several actinides, including isotopes of uranium, neptunium, plutonium and curium was possible. The observed radionuclide composition of the fallout and the time course of ground deposition and air concentration at the site of the Gesellschaft fuer Strahlen- und Umweltforschung (GSF) at Neuherberg, 10 km north of Munich, are reported and discussed. (orig.)

  6. Synthesis of radiopharmaceuticals containing short-lived radionuclides: Comprehensive progress report, March 1, 1986-February 28, 1989

    International Nuclear Information System (INIS)

    Kabalka, G.W.

    1988-06-01

    The primary objective of the DOE Nuclear Medicine Program at The University of Tennessee is the creation of new methods for intoducing short-lived isotopes into agents for use in PET and SPECT. A portion of our effort is directed toward the design and in vivo quantitation of boron-containing neutron therapy agents. The uniqueness of the program is its focus on the design of new chemistry (molecular architecture) and technology as opposed to the application of known reactions to the synthesis of specific radiopharmaceuticals. The following topics are outlined in this paper: new isotope incorporation reactions utilizing nitrogen 13, oxygen 15, and carbon 11; technetium-boron complexes; boron-neutron-capture

  7. Statistical analysis of fallout radionuclides transfer to paddy-field rice

    International Nuclear Information System (INIS)

    Takahashi, T.; Morisawa, S.; Inoue, Y.

    1996-01-01

    Radionuclides released from nuclear facilities to atmosphere are transported through various pathways in biosphere and cause human exposure. Among these radionuclides transfer pathways, an ingestion of crops containing radionuclides is one of the dominant pathway for human exposure. For the safety assessment of nuclear facilities, it is important to understand the behavior of radionuclides in agricultural environment and to describe them in a mathematical model. In this paper, a statistical model is proposed for estimating the concentration of fallout radionuclides in paddy-field rice, the staple food for Japanese people. For describing behavior of fallout radionuclides in a paddy-field, a dynamic model and a statistical model have been proposed respectively. The model used in this study has been developed assuming that the amount of radionuclides transfer to brown rice (hulled rice) or polished rice through direct deposition of airborne radionuclides (the direct deposition pathway) and root uptake from a paddy soil (the root uptake pathway) are proportional to the deposition flux of radionuclides and concentration of radionuclides in paddy soil respectively. That is, the model has two independent variables; the deposition flux of radionuclides and the concentration of radionuclides in the paddy soil, and has single dependent variable; the concentration of radionuclides in brown rice or polished rice. The regression analysis is applied by using environmental monitoring data. Then the distribution of radionuclides between rice-bran (skin part of rice crop) and polished rice (core part) through both the direct deposition pathway and the root uptake pathway are evaluated by the model. (author)

  8. Upscaling the Use of Fallout Radionuclides in Soil Erosion and Sediment Budget Investigations: Addressing the Challenge

    Directory of Open Access Journals (Sweden)

    D.E. Walling

    2014-09-01

    Full Text Available The application of fallout radionuclides in soil erosion investigations and related sediment budget studies has provided a widely used tool for improving understanding of soil erosion and sediment transfer processes. However, most studies using fallout radionuclides undertaken to date have focussed on small areas. This focus on small areas reflects both the issues addressed and practical constraints associated with sample collection and analysis. Increasing acceptance of the important role of fine sediment in degrading aquatic habitats and in the transfer and fate of nutrients and contaminants within terrestrial and fluvial systems has emphasised the need to consider larger areas and the catchment or regional scale. The need to upscale existing approaches to the use of fallout radionuclides to larger areas represents an important challenge. This contribution provides a brief review of existing and potential approaches to upscaling the use of fallout radionuclides and presents two examples where such approaches have been successfully applied. These involve a national scale assessment of soil erosion rates in England and Wales based on 137Cs measurements and an investigation of the sediment budgets of three small/intermediate-size catchments in southern Italy.

  9. Transport and redistribution of Chernobyl fallout radionuclides by fluvial processes: some preliminary evidence

    International Nuclear Information System (INIS)

    Walling, D.E.; Bradley, S.B.

    1988-01-01

    Several measurements of 137 Cs concentrations in suspended sediment transported by the River Severn during the post-Chernobyl period and in recent channel and floodplain deposits along the river emphasise the potential significance of fluvial processes in the transport and concentration of fallout radionuclides. (author)

  10. Transfer of fallout radionuclides derived from Fukushima NPP accident: 1 year study on transfer of radionuclides through hydrological processes

    Science.gov (United States)

    Onda, Yuichi; Kato, Hiroaki; Patin, Jeremy; Yoshimura, Kazuya; Tsujimura, Maki; Wakahara, Taeko; Fukushima, Takehiko

    2013-04-01

    Previous experiences such as Chernobyl Nuclear Power Plant accident have confirmed that fallout radionuclides on the ground surface migrate through natural environment including soils and rivers. Therefore, in order to estimate future changes in radionuclide deposition, migration process of radionuclides in forests, soils, ground water, rivers should be monitored. However, such comprehensive studies on migration through forests, soils, ground water and rivers have not been conducted so far. Here, we present the following comprehensive investigation was conducted to confirm migration of radionuclides through natural environment including soils and rivers. 1)Study on depth distribution of radiocaesium in soils within forests, fields, and grassland 2)Confirmation of radionuclide distribution and investigation on migration in forests 3)Study on radionuclide migration due to soil erosion under different land use 4)Measurement of radionuclides entrained from natural environment including forests and soils 5)Investigation on radionuclide migration through soil water, ground water, stream water, spring water under different land use 6)Study on paddy-to-river transfer of radionuclides through suspended sediments 7)Study on river-to-ocean transfer of radionuclides via suspended sediments 8)Confirmation of radionuclide deposition in ponds and reservoirs

  11. Alimentary tract absorption (f1 values) for radionuclides in local and regional fallout from nuclear tests.

    Science.gov (United States)

    Ibrahim, Shawki A; Simon, Steven L; Bouville, André; Melo, Dunstana; Beck, Harold L

    2010-08-01

    This paper presents gastrointestinal absorption fractions (f1 values) for estimating internal doses from local and regional fallout radionuclides due to nuclear tests. The choice of f1 values are based on specific circumstances of weapons test conditions and a review of reported f1 values for elements in different physical and chemical states. Special attention is given to fallout from nuclear tests conducted at the Marshall Islands. We make a distinction between the f1 values for intakes of radioactive materials immediately after deposition (acute intakes) and intakes that occur in the course of months and years after deposition, following incorporation into terrestrial and aquatic foodstuffs (chronic intakes). Multiple f1 values for different circumstances where persons are exposed to radioactive fallout (e.g., local vs. regional fallout and coral vs. continental tests) are presented when supportive information is available. In some cases, our selected f1 values are similar to those adopted by the International Commission on Radiological Protection (ICRP) (e.g., iodine and most actinides). However, f1 values for cesium and strontium derived from urine bioassay data of the Marshallese population are notably lower than the generic f1 values recommended by ICRP, particularly for acute intakes from local fallout (0.4 and 0.05 for Cs and Sr, respectively). The f1 values presented here form the first complete set of values relevant to realistic dose assessments for exposure to local or regional radioactive fallout.

  12. Estimated inventory of plutonium and uranium radionuclides for vegetation in aged fallout areas

    International Nuclear Information System (INIS)

    Romney, E.M.; Gilbert, R.O.; Wallace, A.; Kinnear, J.

    1976-02-01

    Data are presented on the contamination of vegetation by 239 Pu, 240 Pu, and other radionuclides in aged fallout areas on the Nevada Test Site (NTS) and the Tonopah Test Range (TTR). Comparisons of soil and vegetation inventory estimates indicate that the standing vegetation contributes an insignificant portion of the total amount of 239-240 Pu present in these aged fallout areas. The amounts of Pu available for vegetation-transport to animals grazing on-site would appear to be relatively small in comparison to the total amounts deposited upon soil. Findings indicate that most of the contaminant found on vegetation probably is attributable to resuspendable materials

  13. Cosmogenic radionuclide 7Be in atmospheric fallouts, weather factors and solar activity

    International Nuclear Information System (INIS)

    Kungurov, F.R.

    2011-11-01

    Key words: 7 Be activity, atmospheric fallouts, solar activity, gamma spectroscopy. Subjects of research: cosmogenic radionuclide 7 Be in atmospheric fallouts and surrounding objects of environment, its migrational distribution connected to solar activity and weather meteorologic parameters of the region studied. Purpose of work: Defining correlation between atmospheric humidity and solar activity with concentration and distribution of cosmogenic radionuclide 7 Be. Methods of research: gamma-spectrometry method of activity measurements. The results obtained and their novelty: Cycle of research works on definition of concentration and migrational distribution of CRN 7 Be in Samarkand region during 2002-2005 was carried out for the first time. Volumetric activity of 7 Be in squat air layer of Samarkand was determined. Average density of 7 Be fallouts for the four years of studies was determined. Qualitative correlation bet ween 7 Be fallouts density variations and solar activity, expressed through Wolf number has been found. Qualitative correlation between 7 Be fallouts density variations and amount of precipitations has been found. Regularity in 7 Be concentration decrease towards north latitudes has been detected. Practical value: Developed scintillation method of 7 Be activity detection in atmospheric fallouts was used in works performed in the framework of republican grants 2F-No 1.2.3, CNT RUz PFNI 2F-No 2.1.39 and ITD-7-024. Methodology was used for the estimation of the velocity of erosion processes in the soils of different regions of Uzbekistan. Methodology is used in the works on 7 Be radioactivity measurements. Degree of embed and economic effectivity: Gained results replenish database on 7 Be isotope distribution on Earth regions and its role in formation of some processes, connected with meteorology, agronomy and radioecology of Samarkand region. Field of application: meteorology, agronomy and radioecology. (author)

  14. Fallout

    International Nuclear Information System (INIS)

    Fradkin, P.L.

    1989-01-01

    When the United States government conducted atmospheric nuclear tests in southern Nevada during the 1950s and early 1960s, radioactive fallout drifted downwind onto citizens. The case of Irene Allen v. The United States of America, filed on August 30, 1979, brought to public awareness the plight of residents of Nevada, Utah, and Arizona. Within the context of the trial, this book provides an overview of the development and atmospheric testing of nuclear weapons by the United States, focusing on Shot Harry, the most radioactive of the 105 atmospheric tests conducted from 1951 to 1962

  15. Increased Concentrations of Short-Lived Decay-Series Radionuclides in Groundwaters Underneath the Nopal I Uranium Deposit at Pena Blanca, Mexico

    Science.gov (United States)

    Luo, S.; Ku, T.; Todd, V.; Murrell, M. T.; Dinsmoor, J. C.

    2007-05-01

    The Nopal I uranium ore deposit at Pena Blanca, Mexico, located at > 200 meters above the groundwater table, provides an ideal natural analog for quantifying the effectiveness of geological barrier for isolation of radioactive waste nuclides from reaching the human environments through ground water transport. To fulfill such natural analog studies, three wells (PB1, PB2, and PB3 respectively) were drilled at the site from the land surface down to the saturated groundwater zone and ground waters were collected from each of these wells through large- volume sampling/in-situ Mn-filter filtration for analyses of short-lived uranium/thorium-series radionuclides. Our measurements from PB1 show that the groundwater standing in the hole has much lower 222Rn activity than the freshly pumped groundwater. From this change in 222Rn activity, we estimate the residence time of groundwater in PB1 to be about 20 days. Our measurements also show that the activities of short-lived radioisotopes of Th (234Th), Ra (228Ra, 224Ra, 223Ra), Rn (222Rn), Pb (210Pb), and Po (210Po) in PB1, PB2, and PB3 are all significantly higher than those from the other wells near the Nopal I site. These high activities provide evidence for the enrichment of long-lived U and Ra isotopes in the groundwater as well as in the associated adsorbed phases on the fractured aquifer rocks underneath the ore deposit. Such enrichment suggests a rapid dissolution of U and Ra isotopes from the uranium ore deposit in the vadose zone and the subsequent migration to the groundwater underneath. A reactive transport model can be established to characterize the in-situ transport of radionuclides at the site. The observed change of 222Rn activity at PB1 also suggests that the measured high radioactivityies in ground waters from the site isare not an artifact of drilling operations. However, further studies are needed to assess if or to what extent the radionuclide migration is affected by the previous mining activities at

  16. [Comparative analysis of the radionuclide composition in fallout after the Chernobyl and the Fukushima accidents].

    Science.gov (United States)

    Kotenko, K V; Shinkarev, S M; Abramov, Iu V; Granovskaia, E O; Iatsenko, V N; Gavrilin, Iu I; Margulis, U Ia; Garetskaia, O S; Imanaka, T; Khoshi, M

    2012-01-01

    The nuclear accident occurred at Fukushima Dai-ichi Nuclear Power Plant (NPP) (March 11, 2011) similarly to the accident at the Chernobyl NPP (April 26, 1986) is related to the level 7 of the INES. It is of interest to make an analysis of the radionuclide composition of the fallout following the both accidents. The results of the spectrometric measurements were used in that comparative analysis. Two areas following the Chernobyl accident were considered: (1) the near zone of the fallout - the Belarusian part of the central spot extended up to 60 km around the Chernobyl NPS and (2) the far zone of the fallout--the "Gomel-Mogilev" spot centered 200 km to the north-northeast of the damaged reactor. In the case of Fukushima accident the near zone up to about 60 km considered. The comparative analysis has been done with respect to refractory radionuclides (95Zr, 95Nb, 141Ce, 144Ce), as well as to the intermediate and volatile radionuclides 103Ru, 106Ru, 131I, 134Cs, 137Cs, 140La, 140Ba and the results of such a comparison have been discussed. With respect to exposure to the public the most important radionuclides are 131I and 137Cs. For the both accidents the ratios of 131I/137Cs in the considered soil samples are in the similar ranges: (3-50) for the Chernobyl samples and (5-70) for the Fukushima samples. Similarly to the Chernobyl accident a clear tendency that the ratio of 131I/137Cs in the fallout decreases with the increase of the ground deposition density of 137Cs within the trace related to a radioactive cloud has been identified for the Fukushima accident. It looks like this is a universal tendency for the ratio of 131I/137Cs versus the 137Cs ground deposition density in the fallout along the trace of a radioactive cloud as a result of a heavy accident at the NPP with radionuclides releases into the environment. This tendency is important for an objective reconstruction of 131I fallout based on the results of 137Cs measurements of soil samples carried out at

  17. Transport of fallout and reactor radionuclides in the drainage basin of the Hudson River estuary

    International Nuclear Information System (INIS)

    Simpson, H.J.; Linsalata, P.; Olsen, C.R.; Cohen, N.; Trier, R.M.

    1987-01-01

    Fallout plutonium and radiocesium derived from both weapons testing and local reactor releases are found in the water column and sediments of the Hudson River in readily measurable amounts. The history of fallout delivery and dissolved phase runoff from the drainage basin of 80 Sr, 137 Cs, and /sup 239,240/Pu have been extensively documented since the mid-1950s. Sediment and water column concentrations of 134 Cs, 137 Cs, and /sup 239,240/Pu in the Hudson have also been documented since the mid-1960's and are summarized. Since the peak fallout years, substantial portions of the fallout radionuclides in the drainage basin have become unavailable to normal weathering processes as reflected by a measured decrease in the fallout nuclide transport to the waters of the tidal Hudson. Budget calculations indicate that plutonium may be transported into the estuary from the coastal ocean, and that desorption of radiocesium from particles has allowed a substantial fraction of radiocesium to be exported from the Hudson to marine waters. 29 references, 6 figures, 8 tables

  18. Atmospheric fallout radionuclides in peatland from Southern Poland.

    Science.gov (United States)

    Mróz, Tomasz; Łokas, Edyta; Kocurek, Justyna; Gąsiorek, Michał

    2017-09-01

    Two peat profiles were collected in a peat bog located in Southern Poland and their geochronology were determined using 210 Pb, 238,239+240 Pu and 137 Cs radiometric techniques. The 210 Pb chronologies were established using the constant rate of supply model (CRS) and are in good agreement with the Pu isotopes and 137 Cs time markers. Maximum activities of Pu isotopes were found at a depth corresponding to the early 1960s, which is the period characterized by the maximum nuclear weapon tests. The results showed that the 210 Pb method is the most accurate technique for the determination age and accumulation rate of a peat. The next part of this study calculated linear accumulation rates by analyzing 238,239+240 Pu and 137 Cs vertical distributions in the profiles. Activities of fallout isotopes were also measured in plants covering the peatland. The highest activities of 137 Cs and 210 Pb were found in Calluna vulgaris samples, and 239+240 Pu were found only in two samples (C. vulgaris and leaves of Oxycoccus quadripelatus). Copyright © 2017 Elsevier Ltd. All rights reserved.

  19. FORMATION OF THE SHORT-LIVED RADIONUCLIDE 36Cl IN THE PROTOPLANETARY DISK DURING LATE-STAGE IRRADIATION OF A VOLATILE-RICH RESERVOIR

    International Nuclear Information System (INIS)

    Jacobsen, Benjamin; Yin Qingzhu; Matzel, Jennifer; Hutcheon, Ian D.; Ramon, Erick C.; Weber, Peter K.; Krot, Alexander N.; Nagashima, Kazuhide; Ishii, Hope A.; Ciesla, Fred J.

    2011-01-01

    Short-lived radionuclides (SLRs) in the early solar system provide fundamental insight into protoplanetary disk evolution. We measured the 36 Cl- 36 S-isotope abundance in wadalite ( 36 Cl (τ 1/2 ∼ 3 x 10 5 yr) in the early solar system. Its presence, initial abundance, and the noticeable decoupling from 26 Al raise serious questions about the origin of SLRs. The inferred initial 36 Cl abundance for wadalite, corresponding to a 36 Cl/ 35 Cl ratio of (1.81 ± 0.13) x 10 -5 , is the highest 36 Cl abundance ever reported in any early solar system material. The high level of 36 Cl in wadalite and the absence of 26 Al ( 26 Al/ 27 Al ≤ 3.9 x 10 -6 ) in co-existing grossular (1) unequivocally support the production of 36 Cl by late-stage solar energetic particle irradiation in the protoplanetary disk and (2) indicates that the production of 36 Cl, recorded by wadalite, is unrelated to the origin of 26 Al and other SLRs ( 10 Be, 53 Mn) recorded by primary minerals of CAIs and chondrules. We infer that 36 Cl was largely produced by irradiation of a volatile-rich reservoir in an optically thin protoplanetary disk adjacent to the region in which the CV chondrite parent asteroid accreted while the Sun was a weak T Tauri star. Subsequently, 36 Cl accreted into the Allende CV chondrite together with condensed water ices.

  20. Release and Movement of Radionuclides in Soils Contaminated with Fallout Materials from an Underground Thermonuclear Detonation

    Science.gov (United States)

    1962-07-06

    Studies The degree of dissolution of the fallout material in H2 0, HCl, DTPA, CDTA, and EDDHA solutions was investigated by the suspension method...days was: EDDHA >DTPA>CDTA>H 2 0. while after 65 days the order of effect was: CDTA> EDDHA >DTPA>H 20. Portions of gamma ray spectra of the 106 day...the same amounts of radionuclides as did H120. The most abundant radio- nuclide was radiotungsten for H120, DTPA, CDTA, and EDDHA supernatant liquids

  1. Radionuclides fallout on lichens and mosses and their leaching by rain in a forest ecosystem

    International Nuclear Information System (INIS)

    Guillitte, Olivier; Kirchmann, Rene; Gelder, E. van; Hurtgen, Christian

    1990-01-01

    In the framework of the Belgian radioecological surveillance programme around nuclear power plants and of research into the impact of fallout from the nuclear accident of Chernobyl on the Ardennes forests, samples of lichens and mosses were collected and measured for radioactive content. It was observed that there is a larger variation between the samples of the same species than between various species but collected from the same ecological niche. The ecological half-life of radionuclides is also dependent on location of these organisms in the forest biotope. Some suggestions regarding the sampling standards are proposed. (author)

  2. Transfer of fallout radionuclides by Fukushima NPP accident from tree crown to forest ecosystem

    Science.gov (United States)

    Onda, Y.; Kato, H.; Wakahara, T.; Kawamori, A.; Tsujimura, M.

    2011-12-01

    Radioactive contamination has been detected in Fukushima and the neighboring prefectures due to the nuclear accident at Fukushima Daiichi Nuclear Power Plant (NPP) following the earthquake and tsunami on 11 March 2011. The total deposition of radioactive materials in fallout samples for 137Cs ranged from 0.02to >10 M Bq/m2 for Cs-137. Experimental catchments have been established in Yamakiya district, Kawamata Town, Fukushima prefecture, located about 35 km from Fukushima power plant, and designated as the evacuated zone. Approximate Cs-137 fallout in this area is 200-600k Bq/m2. We established 3 forest sites: broad leaf tree forest and two Japanese cedar forest plantation (young and mature). In each site we installed towers of 8-12 meters. Using these towers, we sampled tree leaves, and measure Cs-137 and Cs-134 in the laboratory, and also we have measure Cs-137, Cs-134 content at various height in each forest using a portable High Purity Germanium (HPGe) detector (Ortech; Detective-EX). We also measured the throughfall, stem flow and litter fall inside of the forest. In each site, we establish the 20 m x 20 m plot to monitor the changes of fallout radionuclides through time with the portable HPGe detector. The monitoring is now ongoing but we found significant amount of Cs-134 and Cs-137 has been trapped by cedar forest plantations especially young trees, but not so much in broad leaf trees. The trapped Cs-137 and Cs-134 is then washed by rainfall and found into throughfall. Therefore, in forest ecosystems, the fallout has been still ongoing, and and effective remediation method in forested area (especially cedar plantation) can be removing the trees.

  3. Use of 137Cs and other fallout radionuclide in soil erosion investigations: progress, problems and prospects

    International Nuclear Information System (INIS)

    Walling, D.E.

    1998-01-01

    Accelerated erosion and soil degradation currently represent serious problems for the global environment. Against this background there is a need to assemble reliable information on the rates of soil loss involved. Existing techniques for documenting rates of soil loss possess many limitations and there is increasing interest in the potential for using fallout radionuclides, particularly 137 Cs, to obtain such information. An example of the application of the 137 Cs approach to a cultivated field at Rufford Forest Farm, Nottinghamshire, UK, is presented to illustrate its value. The key advantages of the approach are that it provides a means of assembling retrospective estimates of medium-term (ca. 40 years) rates of soil loss and the spatial pattern of erosion and deposition involved, on the basis of a single site visit. There are, however, currently a number of problems and uncertainties associated with the use of 137 Cs in soil erosion investigations, and these are reviewed and needs for further research identified. Potential developments of the approach, including the use of other fallout radionuclides such as unsupported 210 Pb and 7 Be are also considered. (author)

  4. Selected natural and fallout radionuclides in plant foods around the Kudankulam Nuclear Power Project, India

    International Nuclear Information System (INIS)

    Ross, E. Mahiban; Raj, Y. Lenin; Wesley, S. Godwin; Rajan, M.P.

    2013-01-01

    The activity concentrations of certain radionuclides were quantified in some plant foods cultivated around Kudankulam, where a mega-nuclear power plant is being established. The activity concentrations were found more in the ‘pulses’ group and were the lowest in ‘other vegetable’ category. The annual effective dose was computed based on the activity concentration of radionuclides and it was found to be higher due to the consumption of cereals and pulses. Other vegetables, cereals, pulses and nuts recorded high transfer factors for the radionuclide 228 Ra. Fruits, leafy vegetables, tubers and roots, and palm embryo registered high transfer factors for 226 Ra. Group-wise activity concentration, radiation dose to the public and soil-plant-to-transfer factor are discussed in detail. Highlights: ► Fallout radionuclides ( 90 Sr and 137 Cs) were below the limit of detection. ► 228 Ra activities were higher than 226 Ra activity concentrations. ► ‘Pulses’ group (leguminous grains) was the highest accumulator of radium nuclides. ► 228 Ra transfer factor was higher in few groups while 226 Ra was higher in others.

  5. Quantifying sources of fine sediment supplied to post-fire debris flows using fallout radionuclide tracers

    Science.gov (United States)

    Smith, Hugh; Sheridan, Gary; Nyman, Petter; Child, David; Lane, Patrick; Hotchkis, Michael

    2013-04-01

    The supply of fine sediment and ash has been identified as an important factor contributing to the initiation of runoff-generated debris flows after fire. However, despite the significance of fines for post-fire debris flow generation, no investigations have sought to quantify sources of this material in debris flow affected catchments. In this study, we employ fallout radionuclides (Cs-137, excess Pb-210 and Pu-239,240) as tracers to measure proportional contributions of fine sediment (bank sources to levee and terminal fan deposits formed by post-fire debris flows in two forest catchments in southeastern Australia. While Cs-137 and excess Pb-210 have been widely used in sediment tracing studies, application of Pu as a tracer represents a recent development and was limited to only one catchment. The estimated range in hillslope surface contributions of fine sediment to individual debris flow deposits in each catchment was 22-69% and 32-74%, respectively. No systematic change in the source contributions to debris flow deposits was observed with distance downstream from channel initiation points. Instead, spatial variability in source contributions was largely influenced by the pattern of debris flow surges forming the deposits. Linking the sediment tracing with interpretation of depositional evidence allowed reconstruction of temporal sequences in sediment source contributions to debris flow surges. Hillslope source inputs dominated most elevated channel deposits such as marginal levees that were formed under peak flow conditions. This indicated the importance of hillslope runoff and sediment supply for debris flow generation in both catchments. In contrast, material stored within channels that was deposited during subsequent surges was predominantly channel-derived. The results demonstrate that fallout radionuclide tracers may provide unique information on the changing source contributions of fine sediment during debris flow events.

  6. Urinary excretion of radionuclides from Marshallese exposed to fallout from the 1954 Bravo nuclear test.

    Science.gov (United States)

    Harris, Payne S; Simon, Steven L; Ibrahim, Shawki A

    2010-08-01

    Soon after the Bravo nuclear test at Bikini Atoll in the Marshall Islands on 1 March 1954, urine samples were collected for analysis of excreted radioactivity from native residents exposed to radioactive fallout on two atolls as well as from U.S. military personnel on a third atoll. The earliest acquired samples, obtained by the Los Alamos Scientific Laboratory (LASL), were assayed for various radionuclides and provided the first known measurements of (131)I in urine following exposure to fallout from a nuclear test. Over the course of 1954, many additional samples were collected by the LASL, as well as by the Atomic Energy Commission New York Operations Office's Health and Safety Laboratory and the Naval Radiological Defense Laboratory. Collectively, the groups sampled included Marshallese exposed on Rongelap and Ailinginae Atolls, American military weather observers temporarily resident on Rongerik Atoll, and sailors from the Japanese fishing vessel, the Lucky Dragon. While the bioassay measurement data and individual urine volumes have been crucial to various attempts to assess intakes of radioactivity and the related internal radiation doses among the Marshallese, those data have never been published in any peer-reviewed journal, but have been restricted to agency memoranda, laboratory reports, and summaries in some publications and book chapters. Reconstructions of internal doses to Marshallese in 1954 and in later years have depended on these data and, hence, they have considerable historical importance as well as importance to ongoing health risk projections for Marshallese. This paper presents much of the original data on urine volumes and radioactivity from the various assays of urine for radionuclides, and compares estimates of (131)I intakes made in 1954, 1985, 1987, and 2008.

  7. Estimation of radionuclide ingestion: Lessons from dose reconstruction for fallout from the Nevada Test Site

    International Nuclear Information System (INIS)

    Breshears, D.D.; Whicker, F.W.; Kirchner, T.B.; Anspaugh, L.R.

    1994-01-01

    The United States conducted atmospheric testing of nuclear devices at the Nevada Test Site from 1951 through 1963. In 1979 the U.S. Department of Energy established the Off-Site Radiation Exposure Review Project to compile a data base related to health effects from nuclear testing and to reconstruct doses to public residing off of the Nevada Test Site. This project is the most comprehensive dose reconstruction project to date, and, since similar assessments are currently underway at several other locations within and outside the U.S., lessons from ORERP can be valuable. A major component of dose reconstruction is estimation of dose from radionuclide ingestion. The PATHWAY food-chain model was developed to estimate the amount of radionuclides ingested. For agricultural components of the human diet, PATHWAY predicts radionuclide concentrations and quantities ingested. To improve accuracy and model credibility, four components of model analysis were conducted: estimation of uncertainty in model predictions, estimation of sensitivity of model predictions to input parameters, and testing of model predictions against independent data (validation), and comparing predictions from PATHWAY with those from other models. These results identified strengths and weaknesses in the model and aided in establishing the confidence associated with model prediction, which is a critical component risk assessment and dose reconstruction. For fallout from the Nevada Test Site, by far, the largest internal doses were received by the thyroid. However, the predicted number of fatal cancers from ingestion dose was generally much smaller than the number predicted from external dose. The number of fatal cancers predicted from ingestion dose was also orders of magnitude below the normal projected cancer rate. Several lessons were learned during the study that are relevant to other dose reconstruction efforts

  8. Determining the times and distances of particle transit in a mountain stream using fallout radionuclides

    Science.gov (United States)

    Bonniwell, Everett C.; Matisoff, Gerald; Whiting, Peter J.

    1999-02-01

    Targeting of erosion and pollution control programs is much more effective if the time for fine particles to be transported through a watershed, the travel distance, the proportions of old and new sediment in suspension, and the rate of erosion of the landscape can be estimated. In this paper we present a novel technique for tracing suspended sediment in a mountain stream using fallout radionuclides sorbed to sediment. Atmospherically-delivered 7Be, 210Pb, and 137Cs accumulate in the snowpack, are released with its melting and sorb to fine particulates, a portion of which are carried downslope into stream channels. The half-life of cosmogenic 7Be is short (53.4 days), thus, sediment residing on the stream bed should contain little of the radionuclide. The different signatures of newly delivered sediment from the landscape with its 7Be tag and older untagged sediment from the channel is the basis for the tracing. The total flux of such radionuclides, compared to the inventory in the soil, permits estimates of the rates of erosion of the landscape. Fine suspended particulates in the Gold Fork River, ID, are transported downstream through the drainage in one or more steps having lengths of tens of kilometers. Length of the step decreases from about 60 km near the peak of the hydrograph to about 12 km near baseflow. The percent of sediment in suspension that is `new' (i.e., recently delivered from the landscape) ranges from 96 to 12%. The remaining sediment is resuspended older channel sediment. Residence times for particulates range from 1.6 days, early in the hydrograph at the upper site, to 103 days late in the hydrograph at the lowest elevation location. Rates of erosion of fine sediment calculated from the flux of radionuclides average 0.0023 cm/year. The long distance transport of fine particles suggests that delivery through the Gold Fork drainage to the basin outlet is fairly rapid once particles reach the channel and perhaps is also rapid in similar and

  9. Dynamic performances of the fallout radionuclides in the environment and related health risk evaluation

    International Nuclear Information System (INIS)

    Morisawa, Shinsuke

    2003-01-01

    The framework was developed for evaluating the cancer induction mortality risk due to the prolonged exposure to the fallout Sr-90 in the environment, which was released by the atmospheric nuclear detonation tests, through dietary intake by considering the effect of foods and feeds import to Japan. The risk evaluation framework presented was composed of three sub-models: the model foe evaluation of the global circulation of Sr-90, the model for evaluation of Sr-90 concentration in foods and dietary intake, and the model for the cancer induction mortality risk. The mortality risk by the radiation-induced leukemia was evaluated based on the NUREG/CR-4214 model. The model was applied on the reference Japanese for past half century to evaluate the historical variation of the health risks. The new framework is presented and discussed on their feasibility to apply on the health risk evaluation due to the low-level and prolonged exposure to radionuclides in the environment. The possibility to use some kind of bio-markers are discussed to evaluate the potential health risk in advance before the risk will be actually detected. (author)

  10. Guidelines for Using Fallout Radionuclides to Assess Erosion and Effectiveness of Soil Conservation Strategies

    International Nuclear Information System (INIS)

    2014-06-01

    Soil degradation currently affects 1.9 billion hectares of agricultural land worldwide, and the area of degraded land is increasing rapidly at a rate of 5 to 7 million hectares each year. Most of this degradation is caused by inappropriate and poor land management practices in agriculture and livestock production. Among all degradation processes, including soil acidification, salinization and nutrient mining, soil erosion is by far the most common type of land degradation, accounting for 84% of affected areas, with more than three quarters of the affected surface land area located in developing countries. Current concerns about the impacts of soil erosion on crop productivity and the environment, as well as the deployment of effective soil conservation measures, have generated an urgent need to obtain reliable quantitative data on the extent and actual rates of soil erosion to underpin sustainable soil conservation strategies. The quest for new approaches for assessing soil erosion to complement conventional methods has led to the development of methodologies based on the use of fallout radionuclides (FRNs) as soil erosion tracers. With increasing attention being paid to land degradation worldwide, this publication explains and demonstrates FRN based methods to trace soil movement and to assess soil erosion at different spatial and temporal scales, and to evaluate the effectiveness of soil conservation strategies to ensure sustainable land management in agricultural systems. This publication summarizes the experiences and knowledge gained since the end of the 1990s in the use of FRNs by the IAEA and by scientists from both developed and developing countries involved in IAEA research networks. This publication provides guidance in the application of FRNs to stakeholders involved in sustainable agricultural development

  11. Sediment dynamics during the rainy season in tropical highland catchments of central Mexico using fallout radionuclides

    International Nuclear Information System (INIS)

    Evrard, Olivier; Ayrault, Sophie; Lefevre, Irene; Bonte, Philippe; Nemery, Julien; Gratiot, Nicolas; Duvert, Clement; Prat, Christian; Esteves, Michel; Poulenard, Jerome

    2010-01-01

    Tropical regions are affected by intense soil erosion associated with deforestation, overgrazing, and cropping intensification. This land degradation leads to important on-site (e.g., decrease in soil fertility) and off-site (e.g., reservoir siltation and water pollution) impacts. This study determined the mean soil particle and sediment residence times in soils and rivers of three sub-catchments (3-12 km 2 ) with contrasted land uses (i.e., cropland, forests, and rangelands) draining to a reservoir located in highlands of the trans-volcanic Mexican belt. Calculations were based on rainfall amount and river discharges as well as on fallout radionuclide measurements (Be-7, Cs-137, and Pb-210) conducted on rainfall precipitated samples, soil sampled in the catchments, and suspended sediment collected by automatic samplers in the river during most storms recorded throughout the 2009 rainy season. Calculations using a radionuclide two-box balance model showed that the mean residence time of particles in soils ranged between 5000 ± 1500 and 23, 300 ± 7000 years. In contrast, sediment residence time in rivers was much shorter, fluctuating between 50 ± 30 and 200 ± 70 days. The shortest mean residence times were measured in a hilly catchment dominated by cropland and rangelands, whereas they were the longest in an undulating catchment dominated by forests and cropland. Calculation of the Be-7/excess-Pb-210 in both rainfall and sediment allowed gaining insight on sediment dynamics throughout the rainy season. The first heavy storms of the year exported the bulk of the sediment stock accumulated in the river channel during the previous year. Then, during the rainy season, the two steeper catchments dominated by cropland and rangelands reacted strongly to rainfall. Sediment was indeed eroded and exported from both catchments during single heavy storms on several occasions in 2009. In contrast, the agro-forested catchment with gentler slopes exported sediment at a

  12. Distribution of artificial radionuclides in particle-size fractions of soil on fallout plumes of nuclear explosions.

    Science.gov (United States)

    Kabdyrakova, A M; Lukashenko, S N; Mendubaev, A T; Kunduzbayeva, A Ye; Panitskiy, A V; Larionova, N V

    2018-06-01

    In this paper are analyzed the artificial radionuclide distributions ( 137 Cs, 90 Sr, 241 Am, 239+240 Pu) in particle-size fractions of soils from two radioactive fallout plumes at the Semipalatinsk Test Site. These plumes were generated by a low-yield surface nuclear test and a surface non-nuclear experiment with insignificant nuclear energy release, respectively, and their lengths are approximately 3 and 0,65 km. In contrast with the great majority of similar studies performed in areas affected mainly by global fallout where adsorbing radionuclides such as Pu are mainly associated with the finest soil fractions, in this study it was observed that along both analyzed plumes the highest activity concentrations are concentrated in the coarse soil fractions. At the plume generated by the surface nuclear test, the radionuclides are concentrated mainly in the 1000-500 μm soil fraction (enrichment factor values ranging from 1.2 to 3.8), while at the plume corresponding to the surface non-nuclear test is the 500-250 μm soil fraction the enriched one by technogenic radionuclides (enrichment factor values ranging from 1.1 to 5.1). In addition, the activity concentration distributions among the different soil size fractions are similar for all radionuclides in both plumes. All the obtained data are in agreement with the hypothesis indicating that enrichment observed in the coarse fractions is caused by the presence of radioactive particles resulted from the indicated nuclear tests. Copyright © 2017 Elsevier Ltd. All rights reserved.

  13. The Project on the distribution of fallout radionuclide and their transfer through environment by Fukushima Daiichi NPP accident

    Science.gov (United States)

    Onda, Yuichi; Kato, Hiroaki; Yoshimura, Kazuya; Fukushima, Takehiko; Patin, Jeremy

    2013-04-01

    Radioactive contamination has been detected in Fukushima due to the nuclear accident at Fukushima Daiichi Nuclear Power Plant (NPP) following the earthquake and tsunami on 11 March 2011. Following comprehensive investigation (FMWSE project funded by MEXT, Japan; http://fmwse.suiri.tsukuba.ac.jp/) was conducted to confirm migration of radionuclides through natural environment including soils and rivers. Experimental catchments have been established in Yamakiya district, Kawamata Town, Fukushima prefecture, located about 35 km from Fukushima power plant, and designated as the evacuated zone. Approximate Cs-137 fallout in this area is 200 - 600 kBq/m2. (1) Migration study of radionuclides in natural environment including forests and rivers: 1) Depth distribution of radiocaesium in soils within forests, fields, and grassland, 2) Confirmation of radionuclide distribution and investigation on migration in forests, 3) Study on radionuclide migration due to soil erosion under different land use, 4) Measurement of radionuclides entrained from natural environment including forests and soils. (2) Migration study of radionuclides through hydrological cycle such as soil water, rivers, lakes and ponds, ground water: 1) Investigation on radionuclide migration through soil water, ground water, stream water, spring water under different land use, 2) Study on paddy-to-river transfer of radionuclides through suspended sediments, 3) Study on river-to-ocean transfer of radionuclides via suspended sediments, 4) Confirmation of radionuclide deposition in ponds and reservoirs. The main finding is as follows: 1) Migration of radionuclides to soil water, stream water and ground water was confirmed low at present. On the other hand, concentration of radiocaesium was found approximately 50 kBq/kg in the suspended sediments flowing down the river. 2) Amount of sediments deposited in the tank placed at the end of downstream within the USLE plot was confirmed together with the concentrations of

  14. Radionuclide characterization and associated dose from long-lived radionuclides in close-in fallout delivered to the marine environment at Bikini and Enewetak Atolls

    International Nuclear Information System (INIS)

    Robison, W.L.; Noshkin, V.E.

    1999-01-01

    Between June 1946 and October 1958, Enewetak and Bikini Atolls were used by the US as testing grounds for 66 nuclear devices. The combined explosive yield from these tests was 107 million t (million t TNT equivalents). This testing produced close-in fallout debris that was contaminated with quantities of radioactive fission and particle activated products, and unspent radioactive nuclear fuel that entered the aquatic environment of the atolls. Today, the sediments in the lagoons are reservoirs for tens of TBq of the transuranics and some long-lived fission and activation products. The larger amounts of contamination are associated with fine and coarse sediment material adjacent to the locations of the high yield explosions. Radionuclides are also distributed vertically in the sediment column to various depths in all regions of the lagoons. Concentrations greater than fallout background levels are found in filtered water sampled over several decades from all locations and depths in the lagoons. This is a direct indication that the radionuclides are continuously mobilized to solution from the solid phases. Of particular importance is the fact that the long-lived radionuclides are accumulated to different levels by indigenous aquatic plants and organisms that are used as food by resident people. One might anticipate finding continuous high contamination levels in many of the edible marine organisms from the lagoons, since the radionuclides associated with the sediments are not contained and are available to the different organisms in a relatively shallow water environment. This is not the case. We estimate that the radiological dose from consumption of the edible parts of marine foods at Enewetak and Bikini is presently approximately 0.05% of the total 50-year integral effective dose from all other exposure pathways that include ingestion of terrestrial foods and drinking water, external exposure and inhalation. The total radiological dose from the marine pathway is

  15. Radionuclide characterization and associated dose from long-lived radionuclides in close-in fallout delivered to the marine environment at Bikini and Enewetak Atoll

    International Nuclear Information System (INIS)

    Noshkin, V. E.; Robison, W. L.

    1998-01-01

    Between June 1946 and October 1958, Enewetak and Bikini Atolls were used by the United States as testing grounds for 66 nuclear devices. The combined explosive yield from these tests was 107 Mt (Mt TNT equivalents). This testing produced close-in fallout debris that was contaminated with quantities of radioactive fission and particle activated products, and unspent radioactive nuclear fuel that entered the aquatic environment of the atolls. Today, the sediments in the lagoons are reservoirs for 10's of TBq of the transuranics and some long-lived fission and activation products. The larger amounts of contamination are associated with fine and coarse sediment material adjacent to the locations of the high yield explosions. Radionuclides are also distributed vertically in the sediment column to various depths in all regions of the lagoons. Concentrations greater than fallout background levels are found in filtered water sampled over several decades from all locations and depths in the lagoons. This is a direct indication that the radionuclides are continuously mobilized to solution from the solid phases. Of particular importance is the fact that the long-lived radionuclides are accumulated to different levels by indigenous aquatic plants and organisms that are used as food by resident people. One might anticipate finding continuous high contamination levels in many of the edible marine organisms from the lagoons, since the radionuclides associated with the sediments are not contained and are available to the different organisms in a relatively shallow water environment. This is not the case. We estimate that the radiological dose from consumption of the edible parts of marine foods at Enewetak and Bikini is presently about 0.05% of the total 50-year integral effective dose from all other exposure pathways that include ingestion of terrestrial foods and drinking water, external exposure and inhalation. The total radiological dose from the marine pathway is dominated by

  16. Synthesis and tissue distribution studies of two novel esters of haloperidol and the application of radiolabelling techniques using short-lived radionuclides in the study of the deposition characteristics of suspended aerosol particles

    International Nuclear Information System (INIS)

    Smith, M.F.

    1982-01-01

    In the present work, the Schotten-Baumann reaction conditions were modified to esterify the tertiary hydroxyl group of haloperidol. The rapid synthesis (less than 20 min) makes this procedure applicable to the preparation of esters of haloperidol containing fluorine-18 (t/sup (1/2)/ 110 min), a γ-emitting radioisotope useful in external scintigraphy. In vivo distribution studies of the synthesized tritiated esters and haloperidol in the rat demonstrated that neither ester prodrug achieved overall higher brain concentration levels than haloperidol. In this study, radiotracer techniques were developed to examine parameters that characterize pressurized aerosols designed to utilize insoluble particles suspended in the aerosol formulation. The suspended micro-aggregated bovine albumin microspheres were labelled with iodine-131 (t/sup (1/2)/ 8 days). The techniques developed illustrate the use of short-lived radionuclides for: 1) quantitation of each metered dose; 2) characterization of particle size distribution by the aerosol; and 3) determination of the extent of deposition of the particles in the aerosol and all of its components

  17. Local area distribution of fallout radionuclides from Fukushima Daiichi Nuclear Power Plant determined by autoradiography analysis

    International Nuclear Information System (INIS)

    Sakamoto, Fuminori; Ohnuki, Toshihiko; Kozai, Naofumi; Igarashi, Shosuke; Yamasaki, Shinya; Yoshida, Zenko; Tanaka, Shunichi

    2012-01-01

    The environmental behavior of radioactive Cs in the fallout from the accident of the Fukushima Daiichi Nuclear Power Plant has been studied by measuring its spatial distribution on/in trees, plants, and surface soil beneath the plants using autoradiography analysis. The results of autoradiography analysis showed that radioactive Cs was distributed on the branches and leaves of trees that were present during the accident and that only a small fraction of radioactive Cs was transported to new branches and leaves grown after the accident. Radioactive Cs was present on the grass and rice stubble on the soils, but not in the soils beneath the grass and rice stubble, indicating that the radioactive Cs was deposited on the grass and the rice plant. In addition, the ratio of the radioactive Cs that penetrated into the soil layer by weathering was very small two months after the accident. These results indicate that trees and other plants are the reservoir of the fallout Cs and function to retard the fallout Cs migration with rain water. (author)

  18. Radionuclide distributions in vertical soil cross sections of the Chernobyl NPP 30-kilometer zone along the western fallout track. II. Chernozem

    International Nuclear Information System (INIS)

    Rogozin, Yu.M.; Smirnova, E.A.; Krivokhatskii, A.S.; Bryzgalova, R.V.; Alekseev, V.A.; Avdeev, V.A.; Kuksov, A.A.; Zudova, I.Yu.

    1993-01-01

    Radionuclide distributions in vertical cross sections taken from chernozem in a former garden and tillable field along the western fallout track at distances of 5, 13.5, and 22 km from the fourth block of the Chernobyl NPP are studied. The distributions through the chernozem cross sections are more complicated than those of sandy soil. Although the main mass of radionuclides in the cross sections is concentrated at depths of 0-3 cm, instances are observed where up to 5-15% of the radionuclides penetrate to greater depths

  19. Health and Safety Laboratory environmental quarterly, March 1, 1977--June 1, 1977. [Air pollution in environs of Cu smelter and fallout radionuclides in food chains

    Energy Technology Data Exchange (ETDEWEB)

    Hardy, E.P. Jr.

    1977-07-01

    This report presents current information from the HASL environmental programs, The Technical University of Wroclaw, Poland, and the Radiological and Environmental Research Division of Argonne National Laboratory. The initial section consists of interpretive reports and notes on environmental levels of lead and mercury in the area of a copper smelter, radionuclide uptake by cultivated dusts in crops, and fallout strontium-90 in diet through 1976. Subsequent sections include tabulations of radionuclide concentrations in stratospheric air, radionuclide and stable lead concentrations in surface air, strontium-90 in deposition, milk, diet, and tapwater and cesium-137 in diet and tapwater. A bibliography of recent publications related to environmental studies is also presented.

  20. Analysis of fresh fallout from Chinese tests by beta counting technique

    International Nuclear Information System (INIS)

    Mishra, U.C.; Lalit, B.Y.; Shukla, V.K.; Ramachandran, T.V.

    1979-01-01

    The paper describes beta counting techniques used in the analysis of fresh radioactive fallout samples from nuclear weapon tests. Fresh fallout samples have been collected by swiping the exposed portion of the engine covers of commercial aircrafts arriving at Bombay from New York after Chinese tests on September 26, 1976 and September 17, 1977. Activities of short-lived radionuclides such as Ag 111, Sr 89, Mo 99, U 237 and Np 239 were determined using these techniques. The results obtained from this analysis is discussed in brief in relation to the kind of fissile material, the extent of thermonuclear reaction in the weapon and the mode of detonation. (orig.) [de

  1. Selected natural and fallout radionuclides in plant foods around the Kudankulam Nuclear Power Project, India.

    Science.gov (United States)

    Ross, E Mahiban; Raj, Y Lenin; Wesley, S Godwin; Rajan, M P

    2013-01-01

    The activity concentrations of certain radionuclides were quantified in some plant foods cultivated around Kudankulam, where a mega-nuclear power plant is being established. The activity concentrations were found more in the 'pulses' group and were the lowest in 'other vegetable' category. The annual effective dose was computed based on the activity concentration of radionuclides and it was found to be higher due to the consumption of cereals and pulses. Other vegetables, cereals, pulses and nuts recorded high transfer factors for the radionuclide (228)Ra. Fruits, leafy vegetables, tubers and roots, and palm embryo registered high transfer factors for (226)Ra. Group-wise activity concentration, radiation dose to the public and soil-plant-to-transfer factor are discussed in detail. Copyright © 2012 Elsevier Ltd. All rights reserved.

  2. Transport of fallout and reactor radionuclides in the drainage basin of the Hudson River estuary

    International Nuclear Information System (INIS)

    Simpson, H.J.; Linsalata, P.; Olsen, C.R.

    1982-01-01

    The transport and fate of Strontium 90, Cesium 137 and Plutonium 239, 240 in the Hudson River Estuary is discussed. Rates of radionuclide deposition and accumulation over time and space are calculated for the Hudson River watershed, estuary, and continental shelf offshore. 37 references, 7 figures, 15 tables

  3. Mass extraction rates of radionuclides in fallout material from a 170-kt nuclear crater

    Energy Technology Data Exchange (ETDEWEB)

    Fleming, E H [Lawrence Radiation Laboratory, University of California, Livermore, CA (United States)

    1969-07-01

    The quantity k is defined as the fraction of a nuclide in the environment which must be ingested each day over a given time period to receive a maximum allowable dose, in accordance with the International Commission on Radiological Protection guidelines. Values of k were computed for radionuclides produced in a single cratering detonation using current design technology. A new concept, called the 'Mass Extraction Rate,' is presented. This concept is defined as the mass of earth material from which the entire quantity of the radionuclide must be extracted and ingested each day by some natural process over a given time interval, which results in a permissible dose. Mass Extraction Rate values are tabulated. A comparison is made between the Mass Extraction Rate and the specific activity methods. (author)

  4. Mass extraction rates of radionuclides in fallout material from a 170-kt nuclear crater

    International Nuclear Information System (INIS)

    Fleming, E.H.

    1969-01-01

    The quantity k is defined as the fraction of a nuclide in the environment which must be ingested each day over a given time period to receive a maximum allowable dose, in accordance with the International Commission on Radiological Protection guidelines. Values of k were computed for radionuclides produced in a single cratering detonation using current design technology. A new concept, called the 'Mass Extraction Rate,' is presented. This concept is defined as the mass of earth material from which the entire quantity of the radionuclide must be extracted and ingested each day by some natural process over a given time interval, which results in a permissible dose. Mass Extraction Rate values are tabulated. A comparison is made between the Mass Extraction Rate and the specific activity methods. (author)

  5. Long-term study on the behaviour of Chernobyl fallout radionuclides in soil

    International Nuclear Information System (INIS)

    Krouglov, S.; Alexakhin, R.; Arkhipov, N.

    1996-01-01

    The evolution with time chemical species of 90 Sr, 106 Ru, 134 Cs, 137 Cs, 144 Ce in soil, and the data on variation of 90 Sr, 134 Cs, 137 Cs transfer to grain and straw of four cereal crops has been used to estimate the rate of radionuclide release from fuel particles and cesium fixation in the soil. Field experiments were carried out in the 30-km restricted zone around Chernobyl NPP

  6. Air concentrations of Chernobyl fallout radionuclides in the area Debrecen (Hungary)

    International Nuclear Information System (INIS)

    Daroczy, S.; Dezsoe, Z.; Pazsit, A.; Buczko, Cs.M.; Somogyi, A.; Papp, Z.; Bolyos, A.; Nagy, J.; Raics, P.

    1991-01-01

    Measurements of aerosol activity from the Chernobyl reactor accident are reported. The concentrations of 14 radionuclides were obtained by gamma spectrometry for the period 30 April - 9 May, 1986. Gross beta measurements were also done through 11 August 1986 of which 137 Cs activity concentrations were derived. 90 Sr activity concentrations were also determined for selected aerosol samples using nondestructive procedure. The time course of contamination observed in Debrecen (Hungary) is discussed in terms of trajectory analysis. Isotopic ratios are also used to trace down routes of contamined air. In addition, such ratios are also used to characterize the status of the damaged reactor at different times. (author) 15 refs.; 2 figs

  7. Tracing the sources of fine sediment in a nickel mining catchment using fallout and geogenic radionuclides (Thio River, New Caledonia)

    Science.gov (United States)

    Evrard, Olivier; Navratil, Oldrich; Lefèvre, Irène; Laceby, J. Patrick; Allenbach, Michel

    2016-04-01

    Soil erosion and subsequent sediment transfer in rivers are exacerbated in tropical regions exposed to heavy rainfall. In New Caledonia, an island located in the southwestern part of the Southern Pacific Ocean, a significant fraction of this sediment is likely originating from tributaries draining nickel mining sites that are known to increase the terrigenous inputs to the rivers and, potentially to UNESCO World Heritage listed coastal lagoons. However, downstream contributions from these tributaries remain to be quantified. A pilot sediment tracing study has therefore been conducted in the 400-km² Thio River catchment. Fallout and geogenic radionuclides have been measured in sediment deposits collected in potential sources, i.e. (i) tributaries draining mines, (ii) tributaries draining 'natural' areas affected by landslides, and (iii) the main stem of the Thio River. Thorium-228 and Caesium-137 provide the best discrimination between sediment originating from the two tributaries. A distribution modelling approach was used to quantify the relative sediment contributions from these tributaries to the Thio River main stem. Results demonstrate that tributaries draining mining sites supply the majority of sediment (67-84%) to the main river. In the future, the validity of these results obtained on sediment deposits collected in April and May 2015 should be verified over a longer time period by applying a similar approach to sediment cores collected in the Thio river deltaic plain. Once validated, this method will be applicable to other catchments draining mines in New Caledonia to design appropriate measures to limit sediment supply to the lagoon.

  8. Vertical random variability of the distribution coefficient in the soil and its effect on the migration of fallout radionuclides

    International Nuclear Information System (INIS)

    Bunzl, K.

    2002-01-01

    In the field, the distribution coefficient, K d , for the sorption of a radionuclide by the soil cannot be expected to be constant. Even in a well defined soil horizon, K d will vary stochastically in horizontal as well as in vertical direction around a mean value. The horizontal random variability of K d produce a pronounced tailing effect in the concentration depth profile of a fallout radionuclide, much less is known on the corresponding effect of the vertical random variability. To analyze this effect theoretically, the classical convection-dispersion model in combination with the random-walk particle method was applied. The concentration depth profile of a radionuclide was calculated one year after deposition assuming constant values of the pore water velocity, the diffusion/dispersion coefficient, and the distribution coefficient (K d = 100 cm 3 x g -1 ) and exhibiting a vertical variability for K d according to a log-normal distribution with a geometric mean of 100 cm 3 x g -1 and a coefficient of variation of CV 0.53. The results show that these two concentration depth profiles are only slightly different, the location of the peak is shifted somewhat upwards, and the dispersion of the concentration depth profile is slightly larger. A substantial tailing effect of the concentration depth profile is not perceivable. Especially with respect to the location of the peak, a very good approximation of the concentration depth profile is obtained if the arithmetic mean of the K d -values (K d = 113 cm 3 x g -1 ) and a slightly increased dispersion coefficient are used in the analytical solution of the classical convection-dispersion equation with constant K d . The evaluation of the observed concentration depth profile with the analytical solution of the classical convection-dispersion equation with constant parameters will, within the usual experimental limits, hardly reveal the presence of a log-normal random distribution of K d in the vertical direction in

  9. Recent research involving the transfer of radionuclides to milk

    International Nuclear Information System (INIS)

    Ward, G.M.

    1989-01-01

    The radionuclides in milk, which result from exposure of dairy cows to radioactive fallout, are a major factor in assessment of internal radiation of humans. To evaluate the radionuclide intake of people from fallout-contaminated milk requires information about feed sources and milk distribution. Pasture intake and the shelf-life of milk are important factors in the case of a short-lived radionuclide like 131 I. Large-scale human radiation assessment studies are underway, all of which consider the dairy food chain as a critical component. These include retrospective studies of fallout from nuclear weapons testing at the Nevada site in the 1950s and the impact of the Chernobyl accident on April 26, 1986

  10. Fallout plutonium and natural radionuclides in annual bands of the coral Montastrea annularis, St. Croix, U.S. Virgin Islands

    International Nuclear Information System (INIS)

    Benninger, L.K.; Dodge, R.E.

    1986-01-01

    We have investigated the banded coral Montastrea annularis as a recorder of the history of fallout Pu in surface seawater. Thirty annual growth bands representing growth during 'coral years' 1951-1980, were subsampled from M. annularis collected at St. Croix, U.S. Virgin Islands. sup(239,240)Pu was finite in coral years 1954-1980, and the coral Pu record is very simply related to the fallout history of 90 Sr. Peaks in coral Pu in coral years 1959 and 1964 correspond to fallout peaks in 1959 and 1963, respectively. Peak broadening and time lags in the coral Pu record, as compared to the 90 Sr fallout record are consistent with retention of fallout Pu in surface seawater for about two years (characteristic removal time) during the period of major fallout, and possibly longer thereafter. The simplicity of the coral Pu record and its close correspondence with fallout history suggest that sup(239,240)Pu was incorporated into the coral skeleton with constant discrimination relative to Ca; the effects of speciation and oxidation state upon Pu incorporation are presently unknown. (author)

  11. Fallout radionuclide based techniques for assessing the effectiveness of soil conservation measures in different eroded regions of China

    International Nuclear Information System (INIS)

    Yu Hanqing; Li Yong; Liu Guoqiang; Li Junjie; Nguyen, M.L.; Funk, R.

    2012-01-01

    Using fallout radionuclide techniques (FRN), we investigated the extent of soil erosion and to quantify the beneficial effects of soil conservation measures at four sites (Xichang city in the Yangtze upriver, Yan'an in the Loess Plateau, Fengning in the wind erosion region of northern China, and Baiquan in black soil region of north-eastern China) extending from South West (SW) to North East (NE) China. At the Xichang site of SW-China, the combined use of FRN 137 Cs and 210 Pbex measurements demonstrated that the effectiveness of vegetation species in reducing soil erosion decreased in the following order: shrubs > trees with litter layer > grasses > trees without litter layer. At the Yan'an site of Loess Plateau, sediment production estimated by 137 Cs declined by 49% due to terracing and by 80% due to vegetated (with grass forest) compared to the cultivated hillslopes. Vegetated hillslope with grasses and forest increased soil organic matter (SOM) by 255%, soil available N (AN) by 198%, and soil available P (AP) by 18% while terracing increased SOM by 121%, soil AN by 103%, and soil AP by 162% compared with the entire cultivated hillslope. Both terracing and vegetating hillslopes were found to enhance soil porosity as shown by a decrease in soil bulk density (1.6% and 6.4%, respectively). At the Fengning site, data from 7 Be measurements indicated that four years of no tillage with high crop residues (50 ∼ 56 cm depth) reduced soil erosion by 44% and no tillage with low residues (25 cm depth) reduced soil erosion rates by 33% when compared with conventional tillage practices. At the Baiquan site in NE-China, soil loss as measured by 137 Cs tracer, decreased by 14% due to terracing and by 34% due to contoured tillage. Our results suggested that shrub cover and composite structure of forest and grass are the effective practices to control hillslope erosion in SW-China, while terracing forest-grass structure can greatly reduce soil erosion and improve soil quality

  12. Acute and chronic intakes of fallout radionuclides by Marshallese from nuclear weapons testing at Bikini and Enewetak and related internal radiation doses.

    Science.gov (United States)

    Simon, Steven L; Bouville, André; Melo, Dunstana; Beck, Harold L; Weinstock, Robert M

    2010-08-01

    Annual internal radiation doses resulting from both acute and chronic intakes of all important dose-contributing radionuclides occurring in fallout from nuclear weapons testing at Bikini and Enewetak from 1946 through 1958 have been estimated for the residents living on all atolls and separate reef islands of the Marshall Islands. Internal radiation absorbed doses to the tissues most at risk to cancer induction (red bone marrow, thyroid, stomach, and colon) have been estimated for representative persons of all population communities for all birth years from 1929 through 1968, and for all years of exposure from 1948 through 1970. The acute intake estimates rely on a model using, as its basis, historical urine bioassay data, for members of the Rongelap Island and Ailinginae communities as well as for Rongerik residents. The model also utilizes fallout times of arrival and radionuclide deposition densities estimated for all tests and all atolls. Acute intakes of 63 radionuclides were estimated for the populations of the 20 inhabited atolls and for the communities that were relocated during the testing years for reasons of safety and decontamination. The model used for chronic intake estimates is based on reported whole-body, urine, and blood counting data for residents of Utrik and Rongelap. Dose conversion coefficients relating intake to organ absorbed dose were developed using internationally accepted models but specifically tailored for intakes of particulate fallout by consideration of literature-based evidence to choose the most appropriate alimentary tract absorption fraction (f1) values. Dose estimates were much higher for the thyroid gland than for red marrow, stomach wall, or colon. The highest thyroid doses to adults were about 7,600 mGy for the people exposed on Rongelap; thyroid doses to adults were much lower, by a factor of 100 or more, for the people exposed on the populated atolls of Kwajalein and Majuro. The estimates of radionuclide intake and

  13. Assessing soil erosion rates for a large catchment in the Central Highlands of Vietnam using fallout radionuclides

    International Nuclear Information System (INIS)

    Phan Son Hai; Nguyen Thanh Binh; Nguyen Minh Dao; Nguyen Thi Huong Lan; Nguyen Thi Mui; Le Xuan Thang; Phan Quang Trung; Trinh Cong Tu; Tran Tien Dung

    2014-01-01

    Fallout radionuclides Be-7 and Cs-137 were applied to assess soil erosion rates for a 270.5 km 2 catchment with a variety of slope (from 0 o to more than 45 o , crops or vegetation (natural forest, artificial forest, perennial crops, annual crops) and a variety of tillage and soil conservation measures. Soil erosion rates were estimated at 90 areas within the catchment. Each sampling area has at least one feature of the slope, rainfall, crops, farming practice different from others. Soil erosion rates in this region depend significantly on the slope, crops and farming techniques. Averaging over crops, soil erosion rates by slopes 0 - 5 o , 5 - 15 o , 15 - 25 o and 25 - 35 o are 5.0, 12.8, 18.9 and 21.3 t.ha -1 .y -1 , respectively. Forest land has the least soil erosion rates, ranging between 0.5 t.ha -1 .y -1 and 14 t.ha -1 .y -1 depending on the slope. Annual crops land has the highest soil erosion rates, ranging between 6 t.ha -1 .y -1 and 42 t.ha -1 .y -1 when slope varies from < 5 o to 32 o . Perennial crop land has soil erosion rates in the range of 5 t.ha -1 .y -1 and 39 t.ha -1 .y -1 . In areas with the same slope, the soil erosion rate is the highest for cashew plantations, lower for mulberry field and the lowest for tea or coffee plantations. Soil erosion has resulted in losing a significant quantity of plant nutrients such as OM, N, P 2 O 5 and K 2 O every year. Generally, lost nutrient quantities due to soil erosion are proportional to erosion rates. Some areas of annual crop land lost a large amount of nutrients every year, up to 1435 kg OM, 79 kg N, 54 kg P 2 O 5 and 36 kg K 2 O. Similarly, perennial crop lands in this region could lost up to 1736 kg OM, 91 kg N, 66 kg P 2 O 5 and 40 kg K 2 O every year. Owing to soil erosion, the catchment has lost about 211200 tons of surface soil per year during last 50 years, corresponding to the rate of 7.8 t.ha -1 .y -1 . This amount of eroded soil was deposited in drainage of the catchment and in reservoirs

  14. Use of fallout radionuclides ((7)Be, (210)Pb) to estimate resuspension of Escherichia coli from streambed sediments during floods in a tropical montane catchment.

    Science.gov (United States)

    Ribolzi, Olivier; Evrard, Olivier; Huon, Sylvain; Rochelle-Newall, Emma; Henri-des-Tureaux, Thierry; Silvera, Norbert; Thammahacksac, Chanthamousone; Sengtaheuanghoung, Oloth

    2016-02-01

    Consumption of water polluted by faecal contaminants is responsible for 2 million deaths annually, most of which occur in developing countries without adequate sanitation. In tropical aquatic systems, streambeds can be reservoirs of persistent pathogenic bacteria and high rainfall can lead to contaminated soils entering streams and to the resuspension of sediment-bound microbes in the streambed. Here, we present a novel method using fallout radionuclides ((7)Be and (210)Pbxs) to estimate the proportions of Escherichia coli, an indicator of faecal contamination, associated with recently eroded soil particles and with the resuspension of streambed sediments. We show that using these radionuclides and hydrograph separations we are able to characterize the proportion of particles originating from highly contaminated soils and that from the resuspension of particle-attached bacteria within the streambed. We also found that although overland flow represented just over one tenth of the total flood volume, it was responsible for more than two thirds of the downstream transfer of E. coli. We propose that data obtained using this method can be used to understand the dynamics of faecal indicator bacteria (FIB) in streams thereby providing information for adapted management plans that reduce the health risks to local populations. Graphical Abstract Graphical abstract showing (1) the main water flow processes (i.e. overland flow, groundwater return flow, blue arrows) and sediment flow components (i.e. resuspension and soil erosion, black arrows) during floods in the Houay Pano catchment; (2) the general principle of the method using fallout radionuclide markers (i.e. (7)Be and (210)Pbxs) to estimate E. coli load from the two main sources (i.e. streambed resuspension vs soil surface washoff); and 3) the main results obtained during the 15 May 2012 storm event (i.e. relative percentage contribution of each process to the total streamflow, values in parentheses).

  15. Appendix to Health and Safety Laboratory environmental quarterly, June 1, 1976--September 1, 1976. [Fallout radionuclides and Pb in environment

    Energy Technology Data Exchange (ETDEWEB)

    Hardy, E.P. Jr.

    1976-10-01

    Tabulated data are presented on the content of /sup 90/Sr and /sup 89/Sr in fallout deposited at various world land sites; /sup 90/Sr in milk and drinking water samples from various locations; and the content of Pb in samples of surface air. (CH)

  16. Practical applications of short-lived radioisotopes

    Energy Technology Data Exchange (ETDEWEB)

    NONE

    1963-01-15

    The advantages of the use of short-lived radioisotopes in agriculture, food industry and medicine as well as some industrial uses are discussed. Methods for isotope production in small research reactors and laboratories are presented

  17. PATHWAY: a dynamic foodchain model to predict radionuclide ingestion after fallout deposition. Final report, September 17, 1979-December 31, 1985

    International Nuclear Information System (INIS)

    Whicker, F.W.; Kirchner, T.B.

    1986-01-01

    This paper describes the structure and basis for parameter values of a computerized foodchain transport model for radionuclides. The model, called ''PATHWAY,'' estimates the time-integrated intake by humans of twenty radionuclides after a single deposition of radioactive material from the atmosphere to the landscape. The model solves a set of differential equations to estimate the inventories and concentrations of radionuclides in three soil layers and numerous types of vegetation, animal tissues and animal products as a function of time following a deposition event. Dynamic processes considered in the model include foliar interception, weathering and absorption; plant growth, uptake, harvest and senescence; soil resuspension, percolation, leaching and tillage; radioactive decay; livestock ingestion, absorption, excretion; and etc. An age- and sex-specific human diet is embodied in the model to permit calculation of time-dependent radionuclide ingestion rates, which are then numerically integrated. 3 figs., 10 tabs

  18. Short-lived radiopharmaceuticals for the diagnosis of ocular melanoma

    International Nuclear Information System (INIS)

    Packer, S.; Lambrecht, R.; Atkins, H.L.; Wolf, A.P.

    1974-01-01

    An experimental procedure has been established to evaluate radiopharmaceuticals for the specific purpose of melanoma detection by scintiscanning. By using the Greene melanoma in the hamster several labeled compounds were compared. Specifically the tumor uptake along with detailed analyses of uptake by various parts of the eye and body were determined in a hamster model. Of those short-lived radionuclides investigated 203 Pb-tris was the most promising as a non-invasive localizing agent for ocular melanoma and it should prove effective for ocular scintigraphy. (U.S.)

  19. Inventories of fallout 21Pb and 137Cs radionuclides in moorland and woodland soils around Edinburgh urban area (UK)

    International Nuclear Information System (INIS)

    Likuku, A.S.; Branford, D.; Fowler, D.; Weston, K.J.

    2006-01-01

    Inventories of fallout 21 Pb and 137 Cs have been measured in moorland and woodland soils around the Edinburgh urban area, using a high purity germanium detector. The 21 Pb inventories in moorland soils were relatively uniform, with a mean value of 2520 ± 270 Bq m -2 . The mean 137 Cs inventory in moorland soils varied greatly from 1310 to 2100 Bq m -2 , with a mean value of 1580 ± 310 Bq m -2 . The variability was ascribed mainly to the non-uniform distribution of fallout Chernobyl 137 Cs. The mean 21 Pb and 137 Cs inventories in woodland canopy soils were found to be 3630 ± 380 Bq m -2 and 2510 ± 510 Bq m -2 , respectively. At sites for which both moorland and woodland data were available, the mean inventories provided fairly similar average enhancements of (47 ± 7)% and (46 ± 18)% of 21 Pb and 137 Cs under woodland canopy soils relative to open grassland soils, respectively. The enhancement factors are broadly in line with other independent findings in literature. Enhancement of both 21 Pb and 137 Cs in woodland soils relative to moorland soils is, in part, due to deposition by impaction during air turbulence, wash-off, gravitational settling and deposition during leaf senescence. Results of this study suggest that these processes affect both 21 Pb and 137 Cs carrier aerosols in a similar way

  20. Radionuclides in ground-level air

    International Nuclear Information System (INIS)

    Sinkko, K.

    1987-01-01

    In the air surveillance programme the concentrations of artificial radionuclides are monitored in the air close to the ground to obtain the necessary basic data for estimating the exposure of the Finnish population to fall-out radionuclides and also to detect atmospheric traces of radioactive materials caused by their use or production. Airborne dust is collected on filters with high-volume air samplers and the concentrations of gamma-emitting radionuclides in the air are evaluated. In the first quarter of 1986 only long-lived cesium, caused by earlier atmospheric nuclear explosions was detected. The concentrations of cesium were very low. In January and March a small amount of short-lived, fresh fission and activation products were also observed

  1. Quantifying the sources and the transit times of sediment using fallout radionuclides (7Be, 137Cs, 210Pbxs) in contrasted cultivated catchments across the world

    Science.gov (United States)

    Evrard, O.; Le Gall, M.; Laceby, J. P.; Foucher, A.; Lefèvre, I.; Salvador-Blanes, S.; Morera, S.; Ribolzi, O.

    2017-12-01

    Soil erosion and fine sediment supply to rivers are exacerbated in intensively cultivated catchments. Information on the sediment sources and transit times in rivers is required to improve our understanding of these processes and to guide the implementation of effective conservation measures. Accordingly, natural (7Be, 210Pb) and artificial (137Cs) fallout radionuclide concentrations were measured in overland flow and suspended sediment collected during the erosive season in contrasted cultivated catchments. In Laos, samples were collected in a steep catchment (Houay Pano, 12 km²) covered with cropland and teak plantations during the first flood of the monsoon in 2014. Cropland surface sources dominated the supply of sediment at the upstream sampling location (55%), whereas subsurface sources (channel, landslides) contributed the majority of material at the outlet (60%). Furthermore, the material exported from the catchment mainly consisted of re-suspended sediment. In Central France, the study was conducted in a flat and drained cultivated catchment (Louroux, 25 km²) during a sequence of winter events in 2013-2014 and 2016. Only surface material enriched in 137Cs was found to transit through the river during floods. The results demonstrated the initial re-suspension of material accumulated in the river channel during the first winter flood before the direct supply of sediment recently eroded from the hillslopes during the next events. In Peru, sediment was collected during a series of summer flood events (2017) in a river draining páramos (Ronquillo, 42 km²) that were recently put in cultivation. Preliminary results show that subsurface re-suspended material dominates the exports from this catchment. These results confirmed the utility of coupling continuous river monitoring and fallout radionuclide measurements on sediment collected in both tropical and temperate rivers to better understand sediment dynamics in these endangered habitats. The main challenges

  2. Radioactive fallout

    International Nuclear Information System (INIS)

    Christensen, G.C.

    1976-01-01

    The formation of the fireball following a nuclear or thermonuclear explosion, and its ascent and cooling are described. Local and global fallout are discussed, and the differing behaviour of fallout from the troposphere and stratosphere explained. The monthly and accumulated fallout of sr90 and its distribution in the Northern and Southern hemispheres is used as an illustration. The accumulation of fallout and its distribution and concentration by food chains is also discussed, using Sr 90, Cs 137 and I 131 as examples. (JIW)

  3. Fallout radionuclide-based techniques for assessing the impact of soil conservation measures on erosion control and soil quality: an overview of the main lessons learnt under an FAO/IAEA Coordinated Research Project.

    Science.gov (United States)

    Dercon, G; Mabit, L; Hancock, G; Nguyen, M L; Dornhofer, P; Bacchi, O O S; Benmansour, M; Bernard, C; Froehlich, W; Golosov, V N; Haciyakupoglu, S; Hai, P S; Klik, A; Li, Y; Lobb, D A; Onda, Y; Popa, N; Rafiq, M; Ritchie, J C; Schuller, P; Shakhashiro, A; Wallbrink, P; Walling, D E; Zapata, F; Zhang, X

    2012-05-01

    This paper summarizes key findings and identifies the main lessons learnt from a 5-year (2002-2008) coordinated research project (CRP) on "Assessing the effectiveness of soil conservation measures for sustainable watershed management and crop production using fallout radionuclides" (D1.50.08), organized and funded by the International Atomic Energy Agency through the Joint FAO/IAEA Division of Nuclear Techniques in Food and Agriculture. The project brought together nineteen participants, from Australia, Austria, Brazil, Canada, Chile, China, Japan, Morocco, Pakistan, Poland, Romania, Russian Federation, Turkey, United Kingdom, United States of America and Vietnam, involved in the use of nuclear techniques and, more particularly, fallout radionuclides (FRN) to assess the relative impacts of different soil conservation measures on soil erosion and land productivity. The overall objective of the CRP was to develop improved land use and management strategies for sustainable watershed management through effective soil erosion control practices, by the use of ¹³⁷Cs (half-life of 30.2 years), ²¹⁰Pb(ex) (half-life of 22.3 years) and ⁷Be (half-life of 53.4 days) for measuring soil erosion over several spatial and temporal scales. The environmental conditions under which the different research teams applied the tools based on the use of fallout radionuclides varied considerably--a variety of climates, soils, topographies and land uses. Nevertheless, the achievements of the CRP, as reflected in this overview paper, demonstrate that fallout radionuclide-based techniques are powerful tools to assess soil erosion/deposition at several spatial and temporal scales in a wide range of environments, and offer potential to monitor soil quality. The success of the CRP has stimulated an interest in many IAEA Member States in the use of these methodologies to identify factors and practices that can enhance sustainable agriculture and minimize land degradation. Copyright

  4. Fallout radionuclide-based techniques for assessing the impact of soil conservation measures on erosion control and soil quality: an overview of the main lessons learnt under an FAO/IAEA Coordinated Research Project

    International Nuclear Information System (INIS)

    Dercon, G.; Mabit, L.; Nguyen, M.L.

    2012-01-01

    This paper summarizes key findings and identifies the main lessons learnt from a 5-year (2002-2008) coordinated research project (CRP) on Assessing the effectiveness of soil conservation measures for sustainable watershed management and crop production using fallout radionuclides (D1.50.08), organized and funded by the International Atomic Energy Agency through the Joint FAO/IAEA Division of Nuclear Techniques in Food and Agriculture. The project brought together nineteen participants, from Australia, Austria, Brazil, Canada, Chile, China, Japan, Morocco, Pakistan, Poland, Romania, Russian Federation, Turkey, United Kingdom, United States of America and Vietnam, involved in the use of nuclear techniques and, more particularly, fallout radionuclides (FRN) to assess the relative impacts of the different soil conservation measure on soil erosion and land productivity. The overall objective of the CRP was to develop improved land use and management strategies for sustainable watershed management through effective soil erosion control practices, by the use of 137 Cs (half-life of 30.2 years), 210 Pb ex (half-life of 22.3 years) and 7 Be (half-life of 53.4 days) for measuring soil erosion over several spatial and temporal scales. The environmental conditions under which the different research teams applied the tools based on the use of fallout radionuclides varied considerably - a variety of climates, soils, topographies and land uses. Nevertheless, the achievements of the CRP, as reflected in this overview paper, demonstrate that fallout radionuclide-based techniques are powerful tools to assess soil erosion/deposition at several spatial and temporal scales in a wide range of environments, and offer potential to monitor soil quality. The success of the CRP has stimulated an interest in many IAEA Member States in the use of these methodologies to identify factors and practices that can enhance sustainable agriculture and minimize land degradation. (author)

  5. Semiquantitative diagnosis of cancer using short-lived radionuclides

    Energy Technology Data Exchange (ETDEWEB)

    Inoue, Tomio; Oriuchi, Noboru; Endo, Keigo [Gunma Univ., Maebashi (Japan). School of Medicine

    1997-03-01

    The accuracy and usefulness of semiquantitative diagnoses of SPECT using radiolabeled monoclonal antibodies in patients with colorectal cancer and PET using FDG in patients with recurrent lung cancer were investigated. The tumor to normal tissue count ratio (T/N ratio) was determined with SPECT and compared with the same index (T/N ratio) obtained by measuring radioactivity in tumor and normal tissue of the resected specimens. Significant correlation between SPECT T/N ratios and tissue T/N ratio was observed (r=0.92, p<0.001, n=8). In PET study, standardized uptake value (SUV) was obtained with PET images and assessed the difference in SUV between recurrent tumors and noncancerous lesions. The relationship between the SUV threshold and diagnostic accuracy in differentiating recurrent tumors from post-treatment changes was also assessed. The maximum SUV in recurrent tumor ranged from 3.0 to 25.8 with a mean {+-} s.d. of 11.2 {+-} 5.7 (n=16) and in the noncancerous lesion ranged from 2.0 to 7.5 with a mean {+-} s.d. of 3.5 {+-} 1.8 (n=9). The SUV was significantly higher in the recurrent cancer (P<0.0001). A threshold SUV of 5.0 provided optimal diagnostic accuracy (sensitivity 93.8%, specificity 88.9%, accuracy 92.0%). It was superior to visual interpretation of FDG PET (sensitivity 100%, specificity 55.6%, accuracy 84%). In conclusion, semiquantitative diagnoses with SPECT using radiolabeled monoclonal antibody and PET using FDG were accurate and useful in detecting malignant tumors. (author)

  6. Short-lived radionuclides program at the University of Michigan

    International Nuclear Information System (INIS)

    Wieland, D.M.

    1985-01-01

    The University of Michigan Nuclear Medicine Research Program, from instrumentation design through radiopharmaceutical development to clinical evaluation, is heavily dependent on the availability and use of iodine-123. Research activities at the University of Michigan can be divided into four major areas: instrumentation, radiochemistry, radiopharmaceutical development, and clinical evaluation. In the first category a new single-photon ring tomograph (SPRINT) has been built and is undergoing performance testing. SPRINT has been designed specifically for brain imaging with 123 I-labeled agents. In the area of radiochemistry, a simple radioiodide exchange technique has been developed for the rapid synthesis of 123 I-labeled aromatic compounds. In the radiopharmaceutical arena, a new agent, 123 I-meta-iodobenzyl-guanidine (MIBG), has been developed - the result of an extensive structure-distribution-relationship study. This radiopharmaceutical, a storage analog of norepinephrine, images organs with rich sympathetic innervation such as the heart and spleen. In the Nuclear Medicine Clinic three 123 I-labeled radiopharmaceuticals are undergoing evaluation

  7. Fallout radionuclide-based techniques for assessing the impact of soil conservation measures on erosion control and soil quality: an overview of the main lessons learnt under an FAO/IAEA Coordinated Research Project

    International Nuclear Information System (INIS)

    Dercon, G.; Mabit, L.; Hancock, G.; Nguyen, M.L.; Dornhofer, P.; Bacchi, O.O.S.; Benmansour, M.; Bernard, C.; Froehlich, W.; Golosov, V.N.; Haciyakupoglu, S.; Hai, P.S.; Klik, A.

    2012-01-01

    This paper summarizes key findings and identifies the main lessons learnt from a 5-year (2002–2008) coordinated research project (CRP) on “Assessing the effectiveness of soil conservation measures for sustainable watershed management and crop production using fallout radionuclides” (D1.50.08), organized and funded by the International Atomic Energy Agency through the Joint FAO/IAEA Division of Nuclear Techniques in Food and Agriculture. The project brought together nineteen participants, from Australia, Austria, Brazil, Canada, Chile, China, Japan, Morocco, Pakistan, Poland, Romania, Russian Federation, Turkey, United Kingdom, United States of America and Vietnam, involved in the use of nuclear techniques and, more particularly, fallout radionuclides (FRN) to assess the relative impacts of different soil conservation measures on soil erosion and land productivity. The overall objective of the CRP was to develop improved land use and management strategies for sustainable watershed management through effective soil erosion control practices, by the use of 137 Cs (half-life of 30.2 years), 210 Pb ex (half-life of 22.3 years) and 7 Be (half-life of 53.4 days) for measuring soil erosion over several spatial and temporal scales. The environmental conditions under which the different research teams applied the tools based on the use of fallout radionuclides varied considerably – a variety of climates, soils, topographies and land uses. Nevertheless, the achievements of the CRP, as reflected in this overview paper, demonstrate that fallout radionuclide-based techniques are powerful tools to assess soil erosion/deposition at several spatial and temporal scales in a wide range of environments, and offer potential to monitor soil quality. The success of the CRP has stimulated an interest in many IAEA Member States in the use of these methodologies to identify factors and practices that can enhance sustainable agriculture and minimize land degradation. - Highlights:

  8. Harvard--MIT research program in short-lived radiopharmaceuticals. Progress report, September 1, 1977--April 30, 1978

    International Nuclear Information System (INIS)

    Adelstein, S.J.; Brownell, G.L.

    1978-05-01

    Progress is reported on the following studies: chemistry studies designed to achieve a more complete understanding of the fundamental chemistry of technetium in order to facilitate the design of future radiopharmaceuticals incorporating the radionuclide /sup 99m/Tc; the development of new radiopharmaceuticals intended to improve image quality and lower radiation doses by the use of short-lived radionuclides and disease-specific agents; the development of short-lived positron-emitting radionuclides which offer advantages in transverse section imaging of regional physiological processes; and studies of the toxic effects of particulate radiation

  9. Spatial and temporal dynamics of sediment in contrasted mountainous watersheds (Mexican transvolcanic belt and French Southern Alps) combining river gauging, elemental geochemistry and fallout radionuclides

    Science.gov (United States)

    Evrard, O.; Navratil, O.; Gratiot, N.; Némery, J.; Duvert, C.; Ayrault, S.; Lefèvre, I.; Legout, C.; Bonté, P.; Esteves, M.

    2009-12-01

    In mountainous environments, an excessive fine sediment supply to the rivers typically leads to an increase in water turbidity, contaminant transport and a rapid filling of reservoirs. This situation is particularly problematic in regions where water reservoirs are used to provide drinking water to large cities (e.g. in central Mexico) or where stream water is used to run hydroelectric power plants (e.g. in the French Southern Alps). In such areas, sediment source areas first need to be delineated and sediment fluxes between hillslopes and the river system must be better understood before implementing efficient erosion control measures. In this context, the STREAMS (« Sediment Transport and Erosion Across MountainS ») project funded by the French National Research Agency (ANR) aims at understanding the spatial and temporal dynamics of sediment at the scale of mountainous watersheds (between 500 - 1000 km2) located in contrasted environments. This 3-years study is carried out simultaneously in a volcanic watershed located in the Mexican transvolcanic belt undergoing a subhumid tropical climate, as well as in a sedimentary watershed of the French Southern Alps undergoing a transitional climate with Mediterranean and continental influences. One of the main specificities of this project consists in combining traditional monitoring techniques (i.e. installation of river gauges, turbidimeters and sediment samplers in several sub-catchments) and sediment fingerprinting using elemental geochemistry (measured by Instrumental Neutron Activation Analysis - INAA - and Inductively Coupled Plasma - Mass Spectrometry - ICP-MS) and fallout radionuclides (measured by gamma spectrometry). In the French watershed, geochemical analysis allows outlining different sediment sources (e.g. the contribution of calcareous vs. marl-covered sub-watersheds). Radionuclide ratios (e.g.Be-7/Cs-137) allow identifying the dominant erosion processes occurring within the watershed. Areas mostly

  10. Radioactive fallout

    International Nuclear Information System (INIS)

    Shapiro, C.S.; Harvey, T.F.; Peterson, K.R.

    1985-12-01

    Potential radiation doses from several scenarios involving nuclear attack on an unsheltered United States population are calculated for local, intermediate time scale and long-term fallout. Dose estimates are made for both a normal atmosphere and an atmosphere perturbed by smoke produced by massive fires. A separate section discusses the additional doses from nuclear fuel facilities, were they to be targeted in an attack. Finally, in an appendix the direct effects of fallout on humans are considered. These include effects of sheltering and biological repair of damage from chronic doses. 21 refs., 10 figs., 11 tabs

  11. Separation of short-lived fission products

    International Nuclear Information System (INIS)

    Tamai, Tadaharu; Ohyoshi, Emiko; Ohyoshi, Akira; Kiso, Yoshiyuki; Shinagawa, Mutsuaki.

    1976-01-01

    A rbief review is presented on the various methods of separation available for both gaseous and liquid states, for the separation of short-lived fission products formed by binary fission of neutron irradiated uranium. The means available for gaseous state are the hot atom reaction, the hydride method and on-line mass separation. For liquid state, use can be made of precipitation, ionic or atomic exchange, solvent extraction and paper electrophoresis. Particular reference is made to electrophoretic separation of ions produced by fission in aqueous solution of uranium. The principle of electrophoretic separation and the procedures for separating the element of interest from the other fission products are outlined, with reference made to the results obtained with the method by the present authors. The elements in question are alkalines, alkaline earths, rare earths, halogens, selenium and

  12. Measurements of Short-Lived Fission Isomers

    Science.gov (United States)

    Finch, Sean; Bhike, Megha; Howell, Calvin; Krishichayan, Fnu; Tornow, Werner

    2016-09-01

    Fission yields of the short lived isomers 134mTe (T1 / 2 = 162 ns) and 136mXe (T1 / 2 = 2 . 95 μs) were measured for 235U and 238U. The isomers were detected by the γ rays associated with the decay of the isomeric states using high-purity germanium detectors. Fission was induced using both monoenergetic γ rays and neutrons. At TUNL's High-Intensity Gamma-ray Source (HI γS), γ rays of 9 and 11 MeV were produced . Monoenergetic 8 MeV neutrons were produced at TUNL's tandem accelerator laboratory. Both beams were pulsed to allow for precise time-gated spectroscopy of both prompt and delayed γ rays following fission. This technique offers a non-destructive probe of special nuclear materials that is sensitive to the isotopic identity of the fissile material.

  13. Spatial distribution of radionuclides in soil around a coal-fired power plant: lead 210, polonium 210, radium 226, thorium 232, kalium 40 emitted with the fly ash and cesium 137 from the worldwide weapon testing fallout

    Energy Technology Data Exchange (ETDEWEB)

    Bunzl, K.; Hoetzl, H.; Rosner, G.; Winkler, R.

    1984-09-01

    To determine the effect of airborne emissions of radionuclides from coal-fired power plants on the environment, the concentrations of the most important radionuclides were measured in soil samples from the local environments (0.4-5.2 km) as well as in fly ash. The spatial distribution of the radionuclides in the soil did not indicate any significantly increased concentrations in the area downwind of the plant compared to other areas; the ratios lead 210/radium 226 and polonium 210/radium 226 were within the range observed for unaffected soils. The emissions from the plant, though present, are obviously too small to significantly change the natural local distribution pattern of the radionuclides in the soil. A highly significant correlation between potassium 40 and thorium 232 was observed which was independent of the different types of soils found in this area. The concentration of cesium 137 in topsoil, which is the result of worldwide fallout from nuclear weapons testing, varied at some places even within a small distance (approx. 2 km) by up to one order of magnitude. Furthermore, it was observed that the concentration of cesium 137 in soils from cropland was on average a factor of 2 less than in those from grassland. This variability has to be considered in planning monitoring programs around nuclear power plants, which may also release this radionuclide. (A.V.)

  14. Continuous administration of short-lived isotopes for evaluating dynamic parameters

    International Nuclear Information System (INIS)

    Selikson, M.

    1985-01-01

    In this paper it is shown that continuous but varying infusions (specifically, exponential infusions) of a short-lived radionuclide can be used to evaluate a wide range of dynamic parameters. The detector response to exponential infusions is derived. An example of an inert diffusible substrate for evaluating regional flow and a glucose model for evaluating regional metabolic rate are both worked out. The advantages of using exponential infusion methods are discussed

  15. The application of retrospective luminescence dosimetry in areas affected by fallout from the semipalatinsk nuclear test site: an evaluation of potential.

    Science.gov (United States)

    Bailiff, I K; Stepanenko, V F; Göksu, H Y; Jungner, H; Balmukhanov, S B; Balmukhanov, T S; Khamidova, L G; Kisilev, V I; Kolyado, I B; Kolizshenkov, T V; Shoikhet, Y N; Tsyb, A F

    2004-12-01

    Luminescence retrospective dosimetry techniques have been applied with ceramic bricks to determine the cumulative external gamma dose due to fallout, primarily from the 1949 test, in populated regions lying NE of the Semipalatinsk Nuclear Test Site in Altai, Russia, and the Semipalatinsk region, Kazakhstan. As part of a pilot study, nine settlements were examined, three within the regions of highest predicted dose (Dolon in Kazakshstan; Laptev Log and Leshoz Topolinskiy in Russia) and the remainder of lower predicted dose (Akkol, Bolshaya Vladimrovka, Kanonerka, and Izvestka in Kazakshstan; Rubtsovsk and Kuria in Russia) within the lateral regions of the fallout trace due to the 1949 test. The settlement of Kainar, mainly affected by the 24 September 1951 nuclear test, was also examined. The bricks from this region were found to be generally suitable for use with the luminescence method. Estimates of cumulative absorbed dose in air due to fallout for Dolon and Kanonerka in Kazakshstan and Leshoz Topolinskiy were 475 +/- 110 mGy, 240 +/- 60 mGy, and 230 +/- 70 mGy, respectively. The result obtained in Dolon village is in agreement with published calculated estimates of dose normalized to Cs concentration in soil. At all the other locations (except Kainar) the experimental values of cumulative absorbed dose obtained indicated no significant dose due to fallout that could be detected within a margin of about 25 mGy. The results demonstrate the potential suitability of the luminescence method to map variations in cumulative dose within the relatively narrow corridor of fallout distribution from the 1949 test. Such work is needed to provide the basis for accurate dose reconstruction in settlements since the predominance of short-lived radionuclides in the fallout and a high degree of heterogeneity in the distribution of fallout are problematic for the application of conventional dosimetry techniques.

  16. Results of calculations of external gamma radiation exposure rates from fallout and the related radionuclide compositions. Operation Tumbler-Snapper, 1952

    International Nuclear Information System (INIS)

    Hicks, H.G.

    1981-07-01

    This report presents data on calculated gamma radiation exposure rates and ground deposition of related radionuclides resulting from Events that deposited detectable radioactivity outside the Nevada Test Site complex

  17. Inventories of fallout {sup 21}Pb and {sup 137}Cs radionuclides in moorland and woodland soils around Edinburgh urban area (UK)

    Energy Technology Data Exchange (ETDEWEB)

    Likuku, A.S. [School of Physics, University of Edinburgh, James Clerk Maxwell Building, King' s Buildings, Mayfield Road, Edinburgh EH9 3JZ (United Kingdom)]. E-mail: alikuku@temo.bca.bw; Branford, D. [School of Physics, University of Edinburgh, James Clerk Maxwell Building, King' s Buildings, Mayfield Road, Edinburgh EH9 3JZ (United Kingdom); Fowler, D. [Centre for Ecology and Hydrology, Edinburgh, Bush Estate, Penicuik, Midlothian EH26 0QB (United Kingdom); Weston, K.J. [School of GeoSciences, University of Edinburgh, James Clerk Maxwell Building, King' s Buildings, Mayfield Road, Edinburgh EH9 3JZ (United Kingdom)

    2006-07-01

    Inventories of fallout {sup 21}Pb and {sup 137}Cs have been measured in moorland and woodland soils around the Edinburgh urban area, using a high purity germanium detector. The {sup 21}Pb inventories in moorland soils were relatively uniform, with a mean value of 2520 {+-} 270 Bq m{sup -2}. The mean {sup 137}Cs inventory in moorland soils varied greatly from 1310 to 2100 Bq m{sup -2}, with a mean value of 1580 {+-} 310 Bq m{sup -2}. The variability was ascribed mainly to the non-uniform distribution of fallout Chernobyl {sup 137}Cs. The mean {sup 21}Pb and {sup 137}Cs inventories in woodland canopy soils were found to be 3630 {+-} 380 Bq m{sup -2} and 2510 {+-} 510 Bq m{sup -2}, respectively. At sites for which both moorland and woodland data were available, the mean inventories provided fairly similar average enhancements of (47 {+-} 7)% and (46 {+-} 18)% of {sup 21}Pb and {sup 137}Cs under woodland canopy soils relative to open grassland soils, respectively. The enhancement factors are broadly in line with other independent findings in literature. Enhancement of both {sup 21}Pb and {sup 137}Cs in woodland soils relative to moorland soils is, in part, due to deposition by impaction during air turbulence, wash-off, gravitational settling and deposition during leaf senescence. Results of this study suggest that these processes affect both {sup 21}Pb and {sup 137}Cs carrier aerosols in a similar way.

  18. Radionuclide deposition and migration within the Gideaa and Finnsjoen study sites, Sweden: A study of the fallout after the Chernobyl accident

    International Nuclear Information System (INIS)

    Gustafsson, E.; Sundblad, B.; Karlberg, O.; Lampe, S.; Tullborg, E.L.

    1987-12-01

    Radionuclides originating from the Chernobyl accident in April 1986 were deposited over large areas of Sweden. The distribution and migration of the radionuclides during the first months after deposition were measured in a comprehensive survey within two study sites, Gideaa in Aangermanland county and Finnsjoen in Uppland county. The sites are previously investigated in the SKB site characterization programme and well defined regarding geology and hydrology. Radionuclides analysed are: Mn-54, Co-60, Sr-90, Zr-95, Nb-95, Mo-99, Ru-103, Ru-106, Ag-110m, Sb-125, I-131, Cs-134, Cs-136, Cs-137, Ba-140, La-140, Ce-141 and Ce-144. The CS-137 surface activity gave a range of 30-100 kBq/m 2 in Gideaa and 20-40 kBq/m 2 in Finnsjoen. Radionuclide migration is observed in soil profiles, groundwater and rock fissures. An active transport by surface water is also evident from sediment samples. Radionuclides have been absorbed in different types of vegetation. (orig./DG)

  19. Tantalum-178 - a short-lived nuclide for nuclear medicine: development of a potential generator system

    International Nuclear Information System (INIS)

    Neirinckx, R.D.; Jones, A.G.; Davis, M.A.; Harris, G.I.; Holman, B.L.

    1978-01-01

    We describe a chemical separation that may form the basis of a generator system for the short-lived radionuclide Ta-178 (T/sub 1/2/ = 9 min). The parent nuclide W-178 (T/sub 1/2/ = 21.7 days) is loaded on an anion-exchange column and the daughter eluted with a mixture of dilute hydrochloric acid and hydrogen peroxide. The yields of tantalum and the breakthrough of the tungsten parent as a function of the eluting conditions are discussed, and preliminary animal distribution data are presented for various treatments of the eluant solution

  20. Results of calculations of external gamma radiation exposure rates from local fallout and the related radionuclide compositions of two hypothetical 1-MT nuclear bursts. Final report

    International Nuclear Information System (INIS)

    Hicks, H.

    1984-12-01

    This report presents data on calculated gamma radiation exposure rates and local surface deposition of related radionuclides resulting from two hypothetical 1-Mt nuclear bursts. Calculations are made of the debris from two types of bombs: one containing 235 U as a fissionable material (designated oralloy), the other containing 238 U (designated tuballoy). 4 references

  1. A survey of radioactive fallout data in Alaska

    International Nuclear Information System (INIS)

    DePhillips, M.P.

    1995-01-01

    Considerable attention has been directed by the scientific community to assessing the levels and fate of radionuclides in Arctic ecosystems. The following text and tables present available data and discussion of radionuclide fallout in Alaska. A literature search of 23 on-line databases (Table 1) using Alaska, Strontium (Sr), Cesium (Cs), Plutonium (Pu) and Radionuclide as constraint terms responded with 177 possible citations. After eliminating duplicate citations, 31 articles were available: 17 were relevant to the subject matter; the remainder addressed geologic issues. All of the cited literature addressed 137 Cs, 90 Sr and 239,240 Pu as a result of radionuclide fallout from nuclear testing or accidental release

  2. Distribution and inventories of fallout radionuclides (239+24Pu, 137Cs) and 21Pb to study the filling velocity of salt marshes in Donana National Park (Spain)

    International Nuclear Information System (INIS)

    Gasco, C.; Anton, M.P.; Pozuelo, M.; Clemente, L.; Rodriguez, A.; Yanez, C.; Gonzalez, A.; Meral, J.

    2006-01-01

    Within an extensive multinational and multidisciplinary project carried out in Donana National Park (Spain) to investigate its preservation and regeneration, the filling velocity of the salt marshes has been evaluated through the calculation of their average sediment accumulation rates. 239+24 Pu and 137 Cs from weapons testing fallout and total 21 Pb distribution profiles and inventories have been determined in some of the most characteristic zones of the park, namely, the ponds (or 'lucios') and the waterjets (or 'canos'). Plutonium inventories range from 16 to 101 Bq m -2 , 137 Cs values fluctuate between 514 and 3758 Bq m -2 and unsupported 21 Pb values comprise between 124 and 9398 Bq m -2 . Average sedimentation rates range from 3 to 5 mm y -1 (1952-2002). These data are higher than those obtained by carbon dating for the period 6500 AD-present, estimated as 1.5-2 mm y -1 , suggesting an increase in the accumulation of sediments and the alteration of the park's hydrodynamics caused by the re-channeling of the major rivers feeding the salt marshes

  3. How Short-Lived Ikaite Affects Calcite Crystallization

    OpenAIRE

    Besselink, R; Rodriguez-Blanco, JD; Stawski, TM; Benning, LG; Tobler, DJ

    2017-01-01

    The pathways of CaCO3 crystallization are manifold, often involving one or several metastable amorphous or nanocrystalline intermediate phases. The presence of such intermediates is often overlooked, because they are short-lived and/or occur at small molar fractions. However, their occurrence does not just impact the mechanisms and pathways of formation of the final stable CaCO3 phase, but also affects their crystal size, shape, and structure. Here we document the presence of a short-lived in...

  4. Modeling the migration of fallout radionuclides to quantify the contemporary transfer of fine particles in Luvisol profiles under different land uses and farming practices

    International Nuclear Information System (INIS)

    Jagercikova, M.; Balesdent, J.; Cornu, S.; Evrard, O.; Lefevre, I.

    2014-01-01

    Soil mixing and the downward movement of solid matter in soils are dynamic pedological processes that strongly affect the vertical distribution of all soil properties across the soil profile. These processes are affected by land use and the implementation of various farming practices, but their kinetics have rarely been quantified. Our objective was to investigate the vertical transfer of matter in Luvisols at long-term experimental sites under different land uses (cropland, grassland and forest) and different farming practices (conventional tillage, reduced tillage and no tillage). To investigate these processes, the vertical radionuclide distributions of 137 Cs and 210 Pb (xs) were analyzed in 9 soil profiles. The mass balance calculations showed that as much as 91± 9% of the 137 Cs was linked to the fine particles (2 mm). To assess the kinetics of radionuclide redistribution in soil, we modeled their depth profiles using a convection-diffusion equation. The diffusion coefficient represented the rate of bioturbation, and the convection velocity provided a proxy for fine particle leaching. Both parameters were modeled as either constant or variable with depth. The tillage was simulated using an empirical formula that considered the tillage depth and a variable mixing ratio depending on the type of tillage used. A loss of isotopes due to soil erosion was introduced into the model to account for the total radionuclide inventory. All of these parameters were optimized based on the 137 Cs data and were then subsequently applied to the 210 Pb (xs) data. Our results show that the 137 Cs isotopes migrate deeper under grasslands than under forests or croplands. Additionally, our results suggest that the diffusion coefficient decreased with depth and that it remained negligible below the tillage depth at the cropland sites, below 20 cm in the forest sites, and below 80 cm in the grassland sites. (authors)

  5. Rapid determination of strontium radionuclides in plants, fodder and foodstuffs

    International Nuclear Information System (INIS)

    Tait, D.; Haase, G.; Hartmann, R.; Jelinski, M.

    2007-01-01

    The fission yield, the transfer factors in the food chain and the dose coefficient are large for the nuclear fission product Sr-90. The surveillance of Sr-90 in the food chain is therefore important in precautionary radiation protection and in assessing the radiation dose to the public especially after a nuclear incident. Prior to analysis, as it is a pure β-emitter, Sr must be separated from the sample by procedures which, for complex organic samples, are lengthy, laborious and dependent on operator skill. Ubiquitous natural radionuclides and short-lived fission products in samples contaminated with fresh fallout may interfere. Here we describe a fast, reproducible and efficient method for extracting Sr from grass, clover, maize, whole meal rye, baby food, and total diet. The method depends on obtaining an ash free of traces of organic interferences. Sr may be separated from a dilute nitric acid leachate of such ash with a solution of dicyclohexyl-18-crown-6 in chloroform. Interfering radionuclides are removed with a special manganese (IV) oxide (active, precipitated from Merck). Sr is precipitated as carbonate then dispersed in a cocktail for liquid scintillation spectrometry. This allows simultaneous counting of Sr-89 (a short-lived β-emitter in fresh fallout) and Sr-90. The chemical yields of Sr determined with the gamma-emitting Sr-85 tracer are reproducible and greater than 75% in all cases. The sample ashing requires 18 h and the extraction 4.0 to 4.5 h. Thus, a duplicate analysis may be completed within 2 days of receipt of the sample. (orig.)

  6. Short-lived positron emitter labeled radiotracers - present status

    International Nuclear Information System (INIS)

    Fowler, J.S.; Wolf, A.P.

    1982-01-01

    The preparation of labelled compounds is important for the application of positron emission transaxial tomography (PETT) in biomedical sciences. This paper describes problems and progress in the synthesis of short-lived positron emitter ( 11 C, 18 F, 13 N) labelled tracers for PETT. Synthesis of labelled sugars, amino acids, and neurotransmitter receptors (pimozide and spiroperidol tagged with 11 C) is discussed in particular

  7. Measurement of short-lived particles at PETRA

    International Nuclear Information System (INIS)

    Saxon, D.H.

    1987-04-01

    The contribution of PETRA to the measurement of short-lived particles is reviewed with discussion of the detectors and analysis techniques. New results are presented on lifetimes of identified particles and the systematics of b-life measurement outlined. The first application of vertex-tagging to flavour separation is described. (author)

  8. Fast Resonance Raman Spectroscopy of Short-Lived Radicals

    DEFF Research Database (Denmark)

    Pagsberg, Palle Bjørn; Wilbrandt, Robert Walter; Hansen, Karina Benthin

    1976-01-01

    We report the first application of pulsed resonance Raman spectroscopy to the study of short-lived free radicals produced by pulse radiolysis. A single pulse from a flash-lamp pumped tunable dye laser is used to excite the resonance Raman spectrum of the p-terphenyl anion radical with an initial...

  9. Applications of nuclear data on short-lived fission products

    International Nuclear Information System (INIS)

    Rudstam, G.; Aagaard, P.; Aleklett, K.; Lund, E.

    1981-01-01

    The study of short-lived fission products gives information about the nuclear structure on the neutron-rich side of stability. The data are also of interest for various applications both to basic science and to nuclear technology. Some of these applications, taken up by the OSIRIS group at Studsvik, are described in the present contribution. (orig.)

  10. Soot and short-lived pollutants provide political opportunity

    Science.gov (United States)

    Victor, David G.; Zaelke, Durwood; Ramanathan, Veerabhadran

    2015-09-01

    Cutting levels of soot and other short-lived pollutants delivers tangible benefits and helps governments to build confidence that collective action on climate change is feasible. After the Paris climate meeting this December, actually reducing these pollutants will be essential to the credibility of the diplomatic process.

  11. Production and Use of Short-Lived Radioisotopes from Reactors. Vol. II. Proceedings of a Seminar on the Practical Applications of Short-Lived Radioisotopes Produced in Small Research Reactors

    International Nuclear Information System (INIS)

    1963-01-01

    There are many radioisotope applications in which it is important that the radiation should rapidly fall to an insignificant level once the initial intense activity has served its purpose. Such applications include diagnostic tests in medicine, where it is essential to reduce the radiation dose to the patient to a minimum, non-destructive testing methods which must be applied without contaminating the material or product concerned, and repeated routine tests which are possible only if the residual activity from the previous test is negligible. All these applications call for radionuclides whose half- lives are measured in hours or even minutes. Similarly, in the new but increasingly important technique of activation analysis, whereby the quantities of elements present in a material can be determined by irradiating the material in a reactor and assaying the radionuclides produced, the latter are mainly short-lived and must be measured immediately. While the production of long-lived radionuclides can most economically be left to the large reactors at the main radioisotope centres, short-lived isotopes must be produced, or materials activation performed, in a reactor at or near the place of intended use or analysis; this, then, represents one of the most important uses for the large number of small reactors which have been installed in recent years, or will come into operation in the near future, in many parts of the world. Since in many countries the new problems of producing, separating and applying short-lived radioisotopes are being faced for the first time, the International Atomic Energy Agency believed it would be valuable to survey the state of the art by convening an international Seminar on Practical Applications of Short-lived Radioisotopes produced in Small Research Reactors at its Vienna headquarters in November, 1962. This Seminar provided an opportunity for the producers and users of short-lived radioisotopes from many countries to meet and discuss the

  12. Production and Use of Short-Lived Radioisotopes from Reactors. Vol. II. Proceedings of a Seminar on the Practical Applications of Short-Lived Radioisotopes Produced in Small Research Reactors

    Energy Technology Data Exchange (ETDEWEB)

    NONE

    1963-03-15

    There are many radioisotope applications in which it is important that the radiation should rapidly fall to an insignificant level once the initial intense activity has served its purpose. Such applications include diagnostic tests in medicine, where it is essential to reduce the radiation dose to the patient to a minimum, non-destructive testing methods which must be applied without contaminating the material or product concerned, and repeated routine tests which are possible only if the residual activity from the previous test is negligible. All these applications call for radionuclides whose half- lives are measured in hours or even minutes. Similarly, in the new but increasingly important technique of activation analysis, whereby the quantities of elements present in a material can be determined by irradiating the material in a reactor and assaying the radionuclides produced, the latter are mainly short-lived and must be measured immediately. While the production of long-lived radionuclides can most economically be left to the large reactors at the main radioisotope centres, short-lived isotopes must be produced, or materials activation performed, in a reactor at or near the place of intended use or analysis; this, then, represents one of the most important uses for the large number of small reactors which have been installed in recent years, or will come into operation in the near future, in many parts of the world. Since in many countries the new problems of producing, separating and applying short-lived radioisotopes are being faced for the first time, the International Atomic Energy Agency believed it would be valuable to survey the state of the art by convening an international Seminar on Practical Applications of Short-lived Radioisotopes produced in Small Research Reactors at its Vienna headquarters in November, 1962. This Seminar provided an opportunity for the producers and users of short-lived radioisotopes from many countries to meet and discuss the

  13. Radionuclides in terrestrial ecosystems

    International Nuclear Information System (INIS)

    Bocock, K.L.

    1981-01-01

    This report summarizes information on the distribution and movement of radionuclides in semi-natural terrestrial ecosystems in north-west England with particular emphasis on inputs to, and outputs from ecosystems; on plant and soil aspects; and on radionuclides in fallout and in discharges by the nuclear industry. (author)

  14. Radionuclide generators

    International Nuclear Information System (INIS)

    Lambrecht, R.M.

    1983-01-01

    The status of radionuclide generators for chemical research and applications related to the life sciences and biomedical research are reviewed. Emphasis is placed upon convenient, efficient and rapid separation of short-lived daughter radionuclides in a chemical form suitable for use without further chemical manipulation. The focus is on the production of the parent, the radiochemistry associated with processing the parent and daughter, the selection and the characteristic separation methods, and yields. Quality control considerations are briefly noted. The scope of this review includes selected references to applications of radionuclide generators in radiopharmaceutical chemistry, and the life sciences, particularly in diagnostic and therapeutic medicine. The 99 Mo-sup(99m)Tc generator was excluded. 202 references are cited. (orig.)

  15. Passive Mobile Bandwidth Classification Using Short Lived TCP Connections

    OpenAIRE

    Michelinakis, Foivos; Kreitz, Gunnar; Petrocco, Riccardo; Zhang, Boxun; Widmer, Joerg

    2015-01-01

    Consumption of multimedia content is moving from a residential environment to mobile phones. Optimizing Quality of Experience—smooth, quick, and high quality playback—is more difficult in this setting, due to the highly dynamic nature of wireless links. A key requirement for achieving this goal is estimating the available bandwidth of mobile devices. Ideally, this should be done quickly and with low overhead. One challenge is that the majority of connections on mobiles are short-lived TCP con...

  16. Radiochemical Procedures Used at Iaea-Ilmr Monaco for Measuring Artificial Radionuclides Resulting from the Chernobyl Accident

    Science.gov (United States)

    Ballestra, S.; Gastaud, J.; Lopez, J. J.

    The Chernobyl accident which occurred on 26 April 1986 resulted in relatively high levels of radioactive fallout over the major part of Europe. Air filter and precipitation samples enabled us to follow the contamination from the accident. In addition contamination was also monitored in selected environmental samples such as seaweeds, sea water, sediment, soil, suspended matter and biological material from the Mediterranean. All samples were counted on Ge(Li) or Ge(HP) detectors to determine the type and quantity of gamma emitting radionuclides and plutonium, americium and curium isotopes were separated and measured using radiochemical techniques and alpha counting. Increased atmospheric radioactivity from the Chernobyl accident was first detected by observing increased activity levels on air filters taken on April 30, 1986, with maximum activities occurring during 1-3 May. Most of the radionuclides initially measured were short-lived fission products. Cs-137 was one of the predominant isotope in the fallout debris and its deposition at Monaco due to Chernobyl was estimated to be around 1400 Bq m-2, which represents 25-40% of the integrated fallout at this latitude. The deposition of Pu-239+240 was much smaller and was estimated to be around 10 mBq m-2 or only 0.1% of the total deposition from nuclear weapon testing.

  17. Limited BRC rulemaking: Regulatory approach and experience in Texas for short-lived radioactive waste

    International Nuclear Information System (INIS)

    McBurney, Ruth E.; Pollard, Christine G.

    1992-01-01

    In 1987, the Texas Department of Health (TDH) implemented a rule to allow, under certain conditions, wastes containing limited concentrations of short- lived radionuclides (less than 300-day half-life) to be disposed of in Type I sanitary landfills. The rule was based on a technical analysis that demonstrated the degree of safety for approximately 340 m of radioactive waste generated annually in Texas and identified major restrictions and conditions for disposal. TDH's Bureau of Radiation Control staff have been able to maintain an account of licensees utilizing the rule during the past years. Several research and industrial facilities in the state have saved significantly on waste disposal expenses. Public concerns and economic impacts for licensees as well as other regulatory aspects and experiences with the rule are discussed. (author)

  18. Transport of short lived radioactive contaminants with prologed half-lives of daughters through river water

    International Nuclear Information System (INIS)

    Metwally, S.M.; Prohl, G.

    2005-01-01

    One of the main pathways for transporting contaminants to other parts in the environment, are rivers. This work is devoted for deriving and assessment the concentration of soluble radio contaminants along a river at any time after discharge, including the short-lived radionuclides in comparison with the discharge time interval, and prolonged half-life of the produced daughter nuclei. The assumed boundary conditions and deduced formulas can be applied either in case of accidental release or discharge under authority control. The formulas determining the produced daughter nuclei concentration require inequality of the parent and daughter nuclei half-lives. Because of the regional variation of river morphology, the assumed constancy of the flow velocity and dispersion coefficient requires dividing the river path into zones of similar hydrologic characteristics

  19. Radioecological sensitivity. Danish fallout data revisited

    International Nuclear Information System (INIS)

    Nielsen, S.P.; Oehlenschlaeger, M.

    1999-01-01

    Danish fallout data covering four decades are interpreted in terms of radioecological sensitivity. The radioecological sensitivity is the time-integrated radionuclide concentration in an environmental sample from a unit ground deposition (e.g. Bq y kg -1 per Gq m -2 ). The fallout data comprise observed levels of the radionuclides 137 Cs and 90 Sr in precipitation, grass, milk, beef and diet. The data are analysed with different types of radioecological models: traditional UNSCEAR models and more recent dynamic models. The traditional models provide empirical relationships between the annual fallout from precipitation and the annual average levels in grass, milk, beef and diet. The relationships may be derived from spreadsheet calculations. ECOSYS and FARMLAND represent more recent radioecological models, which are available as software for personal computers. These models are more mechanistic and require information on a range of topics, e.g. mode of deposition, nuclide dependent and nuclide independent parameters. The more recent models do not reproduce the fallout data better than the traditional models. But the general features of the more recent models make them suited for prediction of radiological consequences of routine and accidental releases in areas where limited radioecological data are available. The work is part of the NKS/BOK-2.1 project on Important Nordic Food Chains aiming at characterising radioecological sensitivity and variability across the Nordic countries. (au)

  20. Fukushima fallout at Milano, Italy

    International Nuclear Information System (INIS)

    Ioannidou, Alexandra; Manenti, Simone; Luigi Gini,; Groppi, Flavia

    2012-01-01

    The radionuclides 131 I, 137 Cs and 134 Cs were observed in the Milano region (45°) of Italy early after the nuclear accident in Fukushima, Japan. Increased atmospheric radioactivity was observed on an air filter taken on 30 March 2011, while the maximum activity of 467 μBq m −3 for 131 I was recorded at April 3–4, 2011. The first evidence of Fukushima fallout was confirmed with 131 I and 137 Cs measured in precipitation at two sampling sites at Milano on 28 March, 2011, with the concentrations of 131 I and 137 Cs in the rainwater equal to 0.89 Bq L −1 and 0.12 Bq L −1 , respectively. A sample of dry deposition that was collected 9 days after the first rainfall event of 27–28 March, 2011 showed that the dry deposition was more effective in the case of 137 Cs than it was for 131 I, probably because iodine was mainly in gaseous form whereas caesium was rapidly bound to aerosols and thus highly subject to dry deposition. The relatively high observed values of 137 Cs in grass, soil and fresh goat and cow milk samples were probably from Chernobyl fallout and global fallout from past nuclear tests rather than from the Fukushima accident. Finally, a dose assessment for the region of investigation showed clearly that the detected activities in all environmental samples were very far below levels of concern. - Highlights: ► Radioactive plume from Fukushima reactor accident reached Milano, Italy. ► 131 I, 137 Cs and 134 Cs were determined in rainwater, air, soil, grass and milk samples. ► The 134 Cs/ 137 Cs activity ratio values in air was about 1. ► High observed values of 137 Cs in grass, soil and milk samples are not due to Fukushima accident. ► The dose assessment show that the observed activities are very far below levels of concern.

  1. Fallout total. beta. radioactivity in every rainfall in Aichi prefecture

    Energy Technology Data Exchange (ETDEWEB)

    Ohnuma, Shoko; Chaya, Kunio; Shimizu, Michihiko; Tomita, Ban-ichi; Hamamura, Norikatsu (Aichi Prefectural Inst. of Public Health, Nagoya (Japan))

    1983-01-01

    Fallout total ..beta.. radioactivity was measured in every rainfall in the period from 1962 to 1981. Maximum value of monthly fallout was 462 mCi/km/sup 2/ at May 1966. Considering changes of monthly fallout, it was assumed that these 20 years were divided to 3 periods and these changes reflected the history of nuclear explosion tests in the world. Maximum value of annual fallout was 1,154 mCi/km/sup 2/ in 1963. Average of annual fallout in 1973 to 1981 was about 1/40 of maximum value. It was confirmed that changes of annual fallout were almost corresponded with changes of annual deposition of /sup 90/Sr and /sup 137/Cs in Tokyo reported by Katsuragi et al. Estimating the staying time of /sup 90/Sr and /sup 137/Cs at Stratosphere by the use of annual fallout of total ..beta.. radioactivity and annual deposition of these radionuclides, /sup 90/Sr was 1.3 years and /sup 137/Cs was 1.5 years. Also, annual correlation between monthly fallout and monthly rainfall was regarded as significant in only 6 years of these 20 years.

  2. Fallout total β radioactivity in every rainfall in Aichi prefecture

    International Nuclear Information System (INIS)

    Ohnuma, Shoko; Chaya, Kunio; Shimizu, Michihiko; Tomita, Ban-ichi; Hamamura, Norikatsu

    1983-01-01

    Fallout total β radioactivity was measured in every rainfall in the period from 1962 to 1981. Maximum value of monthly fallout was 462 mCi/km 2 at May 1966. Considering changes of monthly fallout, it was assumed that these 20 years were divided to 3 periods and these changes reflected the history of nuclear explosion tests in the world. Maximum value of annual fallout was 1,154 mCi/km 2 in 1963. Average of annual fallout in 1973 to 1981 was about 1/40 of maximum value. It was confirmed that changes of annual fallout were almost corresponded with changes of annual deposition of 90 Sr and 137 Cs in Tokyo reported by Katsuragi et al. Estimating the staying time of 90 Sr and 137 Cs at Stratosphere by the use of annual fallout of total β radioactivity and annual deposition of these radionuclides, 90 Sr was 1.3 years and 137 Cs was 1.5 years. Also, annual correlation between monthly fallout and monthly rainfall was regarded as significant in only 6 years of these 20 years. (author)

  3. Harvard-MIT research program in short-lived radiopharmaceuticals. Final report

    International Nuclear Information System (INIS)

    Adelstein, S.J.

    1995-02-01

    The Harvard-MIT Research Program in Short-lived Radiopharmaceuticals was established in 1977 to foster interaction among groups working in radiopharmaceutical chemistry at Harvard Medical School, the Massachusetts Institute of Technology, and the Massachusetts General Hospital. To this was added a group at The Childrens Hospital. From these collaborations and building upon the special strengths of the participating individuals, laboratories and institutions, it was hoped that original approaches would be found for the design of new, clinically useful, radiolabeled compounds. The original thrust of this proposal included: (a) examination of the coordination chemistry of technetium as a basis for rational radiopharmaceutical design, (b) development of an ultrashort-lived radionuclide generator for the diagnosis of congenital heart disease in newborns, (c) synthesis of receptor-site-directed halopharmaceuticals, (d) improved facile labeling of complex molecules with positron-emitting radionuclides. The authors' 1986 proposal was oriented toward organs and disease, emphasizing radiolabeled agents that delineate specific functions and the distribution of receptors in brain, heart, and tumors. In 1989, they further refined their purposes and focused on two major aims: (a) synthesis and utilization of neutral technetium and rhenium complexes of high specific activity, and (b) development of new approaches to the radiolabeling of proteins, peptides, immunoglobulins, and their fragments. In 1992, the authors amended this proposal to concentrate their efforts on biologically active peptides and proteins for targeted radiodiagnosis and therapy

  4. Harvard-MIT research program in short-lived radiopharmaceuticals. Final report

    Energy Technology Data Exchange (ETDEWEB)

    Adelstein, S.J. [Massachusetts Inst. of Tech., Cambridge, MA (United States). Office of Sponsored Programs

    1995-02-01

    The Harvard-MIT Research Program in Short-lived Radiopharmaceuticals was established in 1977 to foster interaction among groups working in radiopharmaceutical chemistry at Harvard Medical School, the Massachusetts Institute of Technology, and the Massachusetts General Hospital. To this was added a group at The Childrens Hospital. From these collaborations and building upon the special strengths of the participating individuals, laboratories and institutions, it was hoped that original approaches would be found for the design of new, clinically useful, radiolabeled compounds. The original thrust of this proposal included: (a) examination of the coordination chemistry of technetium as a basis for rational radiopharmaceutical design, (b) development of an ultrashort-lived radionuclide generator for the diagnosis of congenital heart disease in newborns, (c) synthesis of receptor-site-directed halopharmaceuticals, (d) improved facile labeling of complex molecules with positron-emitting radionuclides. The authors` 1986 proposal was oriented toward organs and disease, emphasizing radiolabeled agents that delineate specific functions and the distribution of receptors in brain, heart, and tumors. In 1989, they further refined their purposes and focused on two major aims: (a) synthesis and utilization of neutral technetium and rhenium complexes of high specific activity, and (b) development of new approaches to the radiolabeling of proteins, peptides, immunoglobulins, and their fragments. In 1992, the authors amended this proposal to concentrate their efforts on biologically active peptides and proteins for targeted radiodiagnosis and therapy.

  5. Real hazards of nuclear fallout

    Energy Technology Data Exchange (ETDEWEB)

    Knox, J.B.; Shapiro, C.S.

    1986-05-01

    The paper discusses an article by Carl Sagan entitled ''On minimizing the consequences of nuclear war'' (Nature 317 485 Oct 1985), in the light of the authors' own work on global fallout. Consequences of local fallout, human impact of local fallout, and global fallout calculations using computer models, are all described. (U.K.).

  6. Are crab-type supernova remnants (plerions) short-lived

    International Nuclear Information System (INIS)

    Weiler, K.W.; Panagia, N.

    1978-01-01

    Arguments are given for a possible picture of the origin, maintenance, and lifetimes of the so-called Crab-like supernova remnants. It is suggested that these objects imply the existence of at least two distinct types of supernova events. A possible connection of the remnant types with the optically defined supernovae of Type I and Type II is discussed. Accepting that a pulsar is formed in at least some supernova events, the proposal is made that a rapidly rotating, rapidly slowing pulsar is necessary to create and maintain a Crab-like supernova remnant. Finally, arguments are presented that such a supernova remnant will be relatively short lived with respect to the more common shell-type of supernova remnant, perhaps surviving only 10000-20000 yr before fading into the Galactic background. The name of plerion is proposed for these filled-center supernova remnants and observational possiblities for confirming their nature are suggested. (orig.) [de

  7. Electron scattering off short-lived radioactive nuclei

    International Nuclear Information System (INIS)

    Wang, S.; Emoto, T.; Furukawa, Y.

    2009-01-01

    We have established a novel method which make electron scattering off short-lived radioactive nuclei come into being. This novel method was named SCRIT (Self-Confining RI ion Target). It was based on the well known "ion trapping" phenomenon in electron storage rings. Stable nucleus, 133 Cs, was used as target nucleus in the R&D experiment. The luminosity of interaction between stored electrons and Cs ions was about 1.02(0.06) × 10 26 cm -2 s -1 at beam current around 80 mA. The angular distribution of elastically scattered electrons from trapped Cs ions was measured. And an online luminosity monitor was used to monitor the change of luminosity during the experiment. (author)

  8. Organic synthesis with short-lived positron-emitting radioisotopes

    International Nuclear Information System (INIS)

    Pike, V.W.

    1988-01-01

    Chemistry with short-lived positron-emitting radioisotopes of the non-metals, principally 11 C, 13 N and 18 F, has burgeoned over the last decade. This has been almost entirely because of the emergence of positron emission tomography (PET) as a powerful non-invasive technique for investigating pathophysiology in living man. PET is essentially an external technique for the rapid serial reconstruction of the spatial distribution of any positron-emitting radioisotope that has been administered in vivo. Such a distribution is primarily governed by the chemical form in which the positron-emitting radioisotope is incorporated, and importantly for clinical research, is often perturbed by physical, biological or clinical factors. Judicious choice of the chemical form enables specific biological information to be obtained. For example, the labelling of glucose with a positron-emitting radioisotope could be expected to provide a radiopharmaceutical for the study of glucose utilisation in both health and disease. (author)

  9. Nondispersive x-ray diagnostics of short lived plasmas

    International Nuclear Information System (INIS)

    Day, R.H.

    1983-01-01

    In this NATO Advanced Study Institute, we have discussed in detail the diagnosis of many pulse power machine properties, including their electrical behavior, grounding and shielding, and related data acquisition techniques. The purpose for many of these machines is to create high temperature/high density plasmas and, therefore, the subsequent behavior of these plasmas is of critical concern. The energy density of these plasmas is such that they will naturally radiate in the x-ray regime and thus the diagnosis of their x-ray emission is a crucial measurement of the entire system performance. In this lecture, I describe the general techniques used to perform nondispersive x-ray diagnostics of these short lived plasmas

  10. Microspheres labelled with short-lived isotopes: Development and application for tumors treatment (Experimental study)

    International Nuclear Information System (INIS)

    Drozdovsky, B.Y.; Rosiev, R.A.; Goncharova, A.Y.; Skvortsov, V.G.; Petriev, V.M.; Grigoriev, A.N.; Schischkanov, N.G.

    1997-01-01

    Analysis of the conducted studies strongly suggests the possibility of usage of the domestic protein microspheres as a vehicle for radionuclide. The neutron-activating method of RPP production enables to utilize a broad spectrum of short-living isotopes that can be delivered into the target organ and anchored there for a long time. Good treatment results were obtained in case of the experimentally induced rheumatoid arthritis in rats after intraarticular loading of 165 Dy-hMSA. Mathematical calculations show that homogeneous distribution of RPP in human articulation cavity with the square of 100 cm 2 can be achieved when the quantity of administered particles exceeds 3000. On the example of 165 Dy-hMSA energy characteristic distribution we demonstrated that the absorbed dose for damaged cells at 2mm distance from the radioactive source is 7 times less than the one for a sphere of 2mm diameter. Analysis of dosimetric data in case of intratumoral loading of 165 Dy-hMSA also point out the necessity of the absorbed dose calculation methods taking into account the distance from the source and possible heterogeneity of RPP distribution inside the tumor to be employed. The prolonged RPP detention in the target causing no essential morphological and functional changes was achieved by embolization on the level of septal and interlobular arteries and of efferent arterioles in the animal's renal. The uniformity of microsphere distribution in the organ and their accumulation in tumors depends on the number of particles being administered. Investigations carried out suggest the efficacy of radionuclide therapy application for treatment of oncological and heavy somatic diseases. They also indicate the necessity of further investigations aimed to optimize the usage of microspheres as a radionuclide carrier usage and to work out the criteria of dosimetric planning

  11. Microspheres labelled with short-lived isotopes: Development and application for tumors treatment (Experimental study)

    Energy Technology Data Exchange (ETDEWEB)

    Drozdovsky, B.Y.; Rosiev, R.A.; Goncharova, A.Y.; Skvortsov, V.G.; Petriev, V.M.; Grigoriev, A.N.; Schischkanov, N.G. [Medical Radiological Research Centre RAMS, Kaluga Region, (Russian Federation)

    1997-10-01

    Analysis of the conducted studies strongly suggests the possibility of usage of the domestic protein microspheres as a vehicle for radionuclide. The neutron-activating method of RPP production enables to utilize a broad spectrum of short-living isotopes that can be delivered into the target organ and anchored there for a long time. Good treatment results were obtained in case of the experimentally induced rheumatoid arthritis in rats after intraarticular loading of {sup 165}Dy-hMSA. Mathematical calculations show that homogeneous distribution of RPP in human articulation cavity with the square of 100 cm{sup 2} can be achieved when the quantity of administered particles exceeds 3000. On the example of {sup 165}Dy-hMSA energy characteristic distribution we demonstrated that the absorbed dose for damaged cells at 2mm distance from the radioactive source is 7 times less than the one for a sphere of 2mm diameter. Analysis of dosimetric data in case of intratumoral loading of {sup 165}Dy-hMSA also point out the necessity of the absorbed dose calculation methods taking into account the distance from the source and possible heterogeneity of RPP distribution inside the tumor to be employed. The prolonged RPP detention in the target causing no essential morphological and functional changes was achieved by embolization on the level of septal and interlobular arteries and of efferent arterioles in the animal`s renal. The uniformity of microsphere distribution in the organ and their accumulation in tumors depends on the number of particles being administered. Investigations carried out suggest the efficacy of radionuclide therapy application for treatment of oncological and heavy somatic diseases. They also indicate the necessity of further investigations aimed to optimize the usage of microspheres as a radionuclide carrier usage and to work out the criteria of dosimetric planning 25 refs.

  12. Radionuclide generators

    International Nuclear Information System (INIS)

    Lambrecht, R.M.; Wollongong Univ.; Tomiyoshi, K.; Sekine, T.

    1997-01-01

    The present status and future directions of research and development on radionuclide generator technology are reported. The recent interest to develop double-neutron capture reactions for production of in vivo generators; neutron rich nuclides for radio-immunotherapeutic pharmaceuticals: and advances with ultra-short lived generators is highlighted. Emphasis is focused on: production of the parent radionuclide; the selection and the evaluation of support materials and eluents with respect to the resultant radiochemical yield of the daughter, and the breakthrough of the radionuclide parent: and, the uses of radionuclide generators in radiopharmaceutical chemistry, biomedical and industrial applications. The 62 Zn → 62 Cu, 66 Ni → 66 Cu, 103m Rh → 103 Rh, 188 W → 188 Re and the 225 Ac → 221 Fr → 213 Bi generators are predicted to be emphasized for future development. Coverage of the 99 Mo → 99m Tc generator was excluded, as it the subject of another review. The literature search ended June, 1996. (orig.)

  13. The contamination of the oceans by anthropogenic radionuclides

    International Nuclear Information System (INIS)

    Figueira, Rubens C.L.; Cunha, Ieda I.L.

    1998-01-01

    Several hundreds of artificial of artificial radionuclides are produced as the result of human activities, such as the applications of nuclear reactors and particle accelerators, testing of nuclear weapons and nuclear accidents. Many of these radionuclides are short-lived and decay quickly after their production, but some of them are longer-lived and are released into the environment. From the radiological point of view the most important radionuclides are cesium-137, strontium-90 and plutonium-239, due to their chemical and nuclear characteristics. The two first radioisotopes present long half life (30 and 28 years), high fission yields and chemical behaviour similar to potassium and calcium, respectively. No stable element exists for plutonium-239, that presents high radiotoxity, longh half-life (24000 years) and some marine organisms accumulate plutonium at high levels. The radionuclides introduced into marine environment undergo various physical, chemical and biological processes taking place in the sea. These processes may be due to physical, dispersion or complicated chemical and biological interactions of the radionuclides with inorganic and organic suspend matter, variety of living organism, bottom sediments, etc. The behaviour of radionuclides in the sea depends primarily on their chemical properties, but it may also be influenced by properties of interacting matrices and other environmental factors. The major route of radiation exposure of man to artificial radionuclides occuring in the marine environment is through ingestion of radiologically contamined marine organisms. This paper summarizes the main sources of contamination in the marine environment and presents an overview covering the oceanic distribution of anthropogenic radionuclides in the FAO regions. A great number of measurements of artificial radioclides have been carried out on various marine environmental samples in different oceans over the world, being cesium-137 the most widely measured

  14. Harvard-MIT research program in short-lived radiopharmaceuticals

    Energy Technology Data Exchange (ETDEWEB)

    Adelstein, S.J.

    1991-01-01

    This report presents research on radiopharmaceuticals. The following topics are discussed: antibody labeling with positron-emitting radionuclides; antibody modification for radioimmune imaging; labeling antibodies; evaluation of technetium acetlyacetonates as potential cerebral blood flow agents; and studies in technetium chemistry. (CBS)

  15. Impact of the Chernobyl fallout in the alpine environment

    International Nuclear Information System (INIS)

    Gastberger, M.; Lettner, H.; Hofmann, W.; Pohl-Rueling, J.; Steinhaeusler, N.F.; Hubmer, A.

    1997-01-01

    In Austria the alpine regions received the highest fallout contamination, showing a very inhomogeneous spatial distribution of the surface deposition. About half of the national territory is within alpine regions, which are very different in times of underlying bedrock and soil characteristic. Since this is the controlling factor for the radionuclide uptake of the vegetation, it is crucial for the long-term effects of radioactive fallout. Different studies have been carried out in the Province of Salzburg (area: 7154 km 2 ) over the past ten years, addressing a broad spectrum of issues, such as: measurement of the spatial distribution of the fallout, research in monitoring techniques comparison of theoretical calculations with actual in vivo-measurements of nuclide uptake by man for different population groups, and the investigation of biological effects. When considering the radioecological effects of the Chernobyl fallout a distinction has to be made between the short-term effects immediately following the fallout and the long-term effects. While the short term effects are controlled by the physical characteristics of the fallout, similar for the whole region, the long-term effects are more determined by the radioecological properties of the environments affected which are much more variable than the fallout-characteristics

  16. Dose estimation from residual and fallout radioactivity, 1

    International Nuclear Information System (INIS)

    Takeshita, Kenji

    1975-01-01

    External dose rates and cumulative doses for early entrants from areal surveys and simulated experiments are reviewed. The average cumulative doses to infinity at the hypocenters were 101 rad in Hiroshima and 32 rad in Nagasaki, with a variation of about 60 percent. Radioactive fallout areas nearly matched the ''black rain'' areas in Nagasaki and in Hiroshima. Radioactivity in the fallout areas was affected by radioactive decay and by the leaching and dissipation by rains. Considering these factors, the cumulative dose to infinity in the fallout area of Hiroshima was estimated to be 13 rad, excluding internal radiation doses from inhaled and ingested radionuclides. Attempts to estimate radiation dose from internally deposited radionuclides are also described. (auth.)

  17. The national scheme for monitoring radioactive fallout in milk

    International Nuclear Information System (INIS)

    Green, B.M.R.

    1979-01-01

    The National Radiological Protection Board, Harwell, assumed responsibility for the national milk monitoring scheme on Jan. 1, 1979. Milk contamination provides a good guide to radioactivity in the British diet. Brief reference is made to U.K. surveys of radioactive fallout in human food prior to January 1979, and current arrangements for the sampling of milk in the U.K. are explained. The milk is analysed for 90 Sr, 137 Cs and stable calcium. Additional samples are collected to check for 131 I or other short-lived isotopes in the event of atmospheric nuclear tests or accidents involving possible releases of radioactivity. (U.K.)

  18. Contribution of short-lived nuclides to decay heat

    International Nuclear Information System (INIS)

    Katakura, Jun-ichi

    1987-01-01

    Comments are made on the calculation of decay heat, centering on evaluation of average decay energy. It is difficult to obtain sufficiently useful decay diagrams of short lived nucleides. High-energy levels are often missing in inferior decay diagrams, leading to an overestimation of the intensity of beta-rays at low-energy levels. Such an overestimation or underestimation due to the inferiority of a decay diagram is referred to as pandemonium effect. The pandemonium effect can be assessed by means of the ratio of the measured energy of the highest level of the daughter nuclide to the Q β -value of the beta-decay. When a satisfactory decay diagram cannot be obtained, the average decay energy has to be estimated by theoretical calculation. The gross theory for beta-decay proposed by Yamada and Takahashi is employed for the calculation. To carry out the calculation according to this theory, it is required to determine the value for the parameter Q 00 , the lowest energy of the daughter nuclide that meets the selection rule for beta-decay. Currently, Q 00 to be used for this purpose is estimated from data on the energy of the lowest level found in a decay diagram, even if it is inferior. Some examples of calculation of decay heat using the average beta- or gamma-ray energy are shown and compared with measurements. (author)

  19. Changing-Look AGNs or Short-Lived Radio Sources?

    Energy Technology Data Exchange (ETDEWEB)

    Wołowska, Aleksandra [Toruń Centre for Astronomy, Faculty of Physics, Astronomy and Informatics, Nicolaus Copernicus University, Toruń (Poland); Kunert-Bajraszewska, Magdalena; Mooley, Kunal [Centre for Astrophysical Surveys, University of Oxford, Oxford (United Kingdom); Hallinan, Gregg, E-mail: ola@astro.umk.pl [Cahill Center for Astronomy, California Institute of Technology, Pasadena, CA (United States)

    2017-11-17

    The evolution of extragalactic radio sources has been a fundamental problem in the study of active galactic nuclei for many years. A standard evolutionary model has been created based on observations of a wide range of radio sources. In the general scenario of the evolution, the younger and smaller Gigahertz-Peaked Spectrum (GPS) and Compact Steep Spectrum (CSS) sources become large-scale FRI and FRII objects. However, a growing number of observations of low power radio sources suggests that the model cannot explain all their properties and there are still some aspects of the evolutionary path that remain unclear. There are indications, that some sources may be short-lived objects on timescales of 10{sup 4}–10{sup 5} years. Those objects represent a new population of active galaxies. Here, we present the discovery of several radio transient sources on timescales of 5–20 yrs, largely associated with renewed AGN (Active Galactic Nucleus) activity. These changing-look AGNs possibly represent behavior typical for many active galaxies.

  20. Emission channeling lattice location experiments with short-lived isotopes

    CERN Multimedia

    Wahl, U; Ronning, C R

    2007-01-01

    Emission channeling with position-sensitive detectors is a well-established technique at ISOLDE for studying the lattice location of radioactive impurities implanted into single crystals. In the case of electron emitting isotopes, however, due to count rate and noise-related limitations of the detection systems, the technique was restricted to isotopes with half lives above 6 h and electron energies above 40 keV. Recently, major technical developments have been realized and new equipment has been acquired which has allowed these limitations to be overcome and made feasible electron emission channeling experiments with short-lived isotopes and at low electron energies.\\\\ As first application, making use of two new on-line emission channeling setups at ISOLDE, we propose to investigate the lattice location of the transition metals Ni (2.5 h) and Co (1.6 h) in semiconductors, in particular in ZnO and GaN, by means of on-line $\\beta^{-}$-emission channeling experiments. In addition, we would like to study the lat...

  1. Quantifying short-lived events in multistate ionic current measurements.

    Science.gov (United States)

    Balijepalli, Arvind; Ettedgui, Jessica; Cornio, Andrew T; Robertson, Joseph W F; Cheung, Kin P; Kasianowicz, John J; Vaz, Canute

    2014-02-25

    We developed a generalized technique to characterize polymer-nanopore interactions via single channel ionic current measurements. Physical interactions between analytes, such as DNA, proteins, or synthetic polymers, and a nanopore cause multiple discrete states in the current. We modeled the transitions of the current to individual states with an equivalent electrical circuit, which allowed us to describe the system response. This enabled the estimation of short-lived states that are presently not characterized by existing analysis techniques. Our approach considerably improves the range and resolution of single-molecule characterization with nanopores. For example, we characterized the residence times of synthetic polymers that are three times shorter than those estimated with existing algorithms. Because the molecule's residence time follows an exponential distribution, we recover nearly 20-fold more events per unit time that can be used for analysis. Furthermore, the measurement range was extended from 11 monomers to as few as 8. Finally, we applied this technique to recover a known sequence of single-stranded DNA from previously published ion channel recordings, identifying discrete current states with subpicoampere resolution.

  2. Radioactive fallout from the Chernobyl nuclear reactor accident

    International Nuclear Information System (INIS)

    Beiriger, J.M.; Failor, R.A.; Marsh, K.V.; Shaw, G.E.

    1987-08-01

    This report describes the detection of fallout in the United States from the Chernobyl nuclear reactor accident. As part of its environmental surveillance program, Lawrence Livermore National Laboratory maintained detectors for gamma-emitting radionuclides. Following the reactor accident, additional air filters were set out. Several uncommon isotopes were detected at the time the plume passed into the US

  3. Synthesis of radiopharmaceuticals containing short-lived radionuclides. Progress report, March 1, 1986-February 28, 1987

    International Nuclear Information System (INIS)

    Kabalka, G.W.

    1986-09-01

    New methods are described for incorporating iodine-123, bromine-75, fluorine-18, oxygen-15, nitrogen-13, and carbon-11 into functionally substituted molecules such as β,β-dimethylsubstituted fatty acids, iodovinyl fatty acids, steroids, amphetamines, alcohols, and other agents of current interest to nuclear medicine researchers. 52 refs

  4. Study of the short-lived fission products. Separation of iodine and xenon fission radionuclides

    International Nuclear Information System (INIS)

    Barrachina, M.; Villar, M. A.

    1965-01-01

    The separation by distillation in a sulfuric acid or phosphoric acid-hydrogen peroxide medium of the iodine isotopes (8 day iodine-131, 2,3 hour iodine-132 21 hour iodine-133, 53 minute iodine-134 and 6,7 hour iodine-135) present in a uranium sample after different irradiation and cooling times is here described. It is also reported the use of active charcoal columns for the retention of xenon isotopes (5,27 days xenon-133 and 9,2 hours xenon-135) either released during the dissolution of the uranium irradiated samples or generated along the fission isobaric chains in the solutions of distillated iodine. In both cases the radiochemical purity of the separated products is established by gamma spectrometry. (Author) 15 refs

  5. Short-lived cyclotron produced radionuclides evaluation on the myocardial imaging agents

    International Nuclear Information System (INIS)

    Rikitake, Tomoyuki; Tateno, Yukio; Yamane, Akiko; Matsumoto, Touru; Umegaki, Youichiro

    1978-01-01

    Organ uptake after venous administration of 13 N-ammonia, 43 K, 86 Rb, 201 Tl and after rectal administration of 13 N-ammonia was studied. Each nuclides highly accumulated in myocardium after intravenous injection, but rectal administrated 13 N-ammonia did not show this tendency. Intravenously injected 13 N-ammonia showed very early myocardial uptake and early secretion from kidney. Rectal administrated 13 N-ammonia was less accumulated in myocardium. 43 KCl and 13 NH 4 Cl were injected intravenously and administrated from the rectum to the rabbits under imaging scintilator system. Whole-body scintiscanner with display-processing unit was used for a 43 KCl injected rabbit. A positroncamera with computer system (TOSBAC 3400 on line system) was used for 13 NH 4 Cl (i.v. and rectal ad.) rabbits. The dynamic studies of 43 KCl, 13 NH 4 Cl were made from these imaging data. The countratio of heart to the liver after 43 K injection was nearly equal or less than the liver. The peakcount was at 15 min after 13 NH 4 Cl intravenous injection. 13 N accumulated promptly at upper mediastinal part and kidney, and soon disappeared from these part. Uptake of the heat was high and that of the liver was low. When 13 NH 4 Cl was administrated from the rectum, 13 N trapped at the liver, and uptake of the heart was very low level. Scintiscanning after 13 KCl intravenously injected, did not show the high resolution. Rabbit heart was distinguishable from the liver, but there are no visibility of the detail. Seeing positronscintigram after 13 NH 4 Cl administration both from intravenously and from rectum, the detail was well visible. We concluded the positron scintigram after 13 NH 4 Cl injection should be a good myocardial imaging agent. Furthermore, 13 Nh 4 Cl has two eminent characters as a myocardial imaging agent comparing 201 TlCl. One is prompt making of image, the others is the very low radiation dose. (auth.)

  6. Position on short-lived radionuclides of the American College of Nuclear Physicians

    International Nuclear Information System (INIS)

    Shoop, J.D.

    1985-01-01

    The more than 1100 nuclear medicine physicians who make up the bulk of the ACNP membership have as their goal the optimum practice of nuclear medicine; hence the purpose of the College as their professional association is to help them achieve this goal, acting primarily in areas where as individuals they cannot work effectively, gathering and disseminating information and other resources, assessing the impact of new technology on practice, combating interference with good practice, enhancing the quality of services offered their patients, and striving to maintain economic stability in the nuclear medicine minisystem

  7. The preparation of organic radiopharmaceuticals and labelled compounds using short-lived cyclotron-produced radionuclides

    International Nuclear Information System (INIS)

    Uhlenhut, G.J.; Koch, H.

    1982-01-01

    Accelerator-produced nuclides and radiopharmaceutical production are discussed with examples of pertinent methods of isotope production, methods of incorporation into organic molecules, and the general problems attandant on the production and use of these materials in this new and interdisciplinary effort. The literature is surveyed with stress being given to the use of 11 C, 13 N and 15 O. 205 references are included. (author)

  8. Rapid radiochemical separation of short-lived radionuclides in neutron-activated samples

    International Nuclear Information System (INIS)

    Fardy, J.

    1985-11-01

    Radiochemical separation procedures based on the removal of metal ions by columns of C 18 -bonded silica gel after selective complexation are examined and the simplicity of the method demonstrated by its application to determination of Mn, Cu and Zn in neutron-activated biological material from the following solutions (pH 0-10, sulphate concentration 0,18M and 1,44M SO 4 ): 8-hydroxyquinoline (oxine), ammonium pyrrolidinedithiocarbamate (APDC), cupferron (CUP), 1-(2-pyridylazo)-2-naphthol (PAN), 1-(2'-thiazolylazo)-2-naphthol (TAN), 4-(2-pyridylazo) resorcinol (PAR), diethylammonium diethyldithiocarbamate (DDC), potassium ethyl xanthate (PEX), acetylacetone (AcAc) or thenoyltrifluoracetone (TTA). The method is rapid and reliable and readily adaptable in all radiochemical laboratories

  9. Short-lived radiopharmaceutical development at E.R. Squibb and Sons, Inc

    International Nuclear Information System (INIS)

    Loberg, M.D.

    1985-01-01

    This paper describes the present status and future plans of E.R. Squibb and Sons, Inc. as they relate to the development of short-lived radiopharmaceuticals. The advantages of short-lived radiopharmaceuticals are summarized as are the problems inherent in their manufacture, quality control, and distribution. The nuclear generator is advocated as the best means of distributing short-lived radiopharmaceuticals. The E.R. Squibb and Sons work with the 82 Sr → 82 Rb generator is summarized

  10. Radioactive fallout in the southern hemisphere from nuclear weapons tests

    International Nuclear Information System (INIS)

    Moroney, J.R.

    1979-11-01

    Fallout in the southern hemisphere, and its origins in the national programs of atmospheric nuclear weapons testing in both hemispheres, are reviewed. Of the 390 nuclear tests conducted in the atmosphere to date, 53 were carried out in the southern hemisphere and it is the second phase of these, between 1966 and 1974, that is seen to have been responsible for the main fallout of short-lived fission products in the southern hemisphere. In contrast to this, the programs of atmospheric nuclear testing in the northern hemisphere up to 1962 are shown to have been the main source of long-lived fission products in fallout in the southern hemisphere. The course followed by this contamination through the environment of the southern hemisphere is traced for the national programs of nuclear testing after 1962 taken separately (France, China) and for the earlier national programs taken together (U.S.S.R., U.S.A. and U.K.). The impact on populations in the southern hemisphere of fallout from atmospheric nuclear weapons tests to date is assessed

  11. Radioactive fallout in the southern hemisphere from nuclear weapons tests

    International Nuclear Information System (INIS)

    Moroney, J.R.

    1979-01-01

    Fallout in the southern hemisphere, and its origins in the national programs of atmospheric nuclear weapons testing in both hemispheres, are reviewed. Of the 390 nuclear tests conducted in the atmosphere to date, 53 were carried out in the southern hemisphere and it is the second phase of these, between 1966 and 1974, that is seen to have been responsible for the main fallout of short-lived fission products in the southern hemisphere. In contrast to this, the programs of atmospheric nuclear testing in the northern hemisphere up to 1962 are shown to have been the main source of long-lived fission products in fallout in the southern hemisphere. The course followed by this contamination through the environment of the southern hemisphere is traced for the national programs of nuclear testing after 1962 taken separately (France, China) and for the earlier national programs taken together (U.S.S.R., U.S.A. and U.K.). The impact on populations in the southern hemisphere of fallout from atmospheric nuclear weapons tests to date is assessed. (author)

  12. Fallout Radioactivity and Epiphytes.

    Science.gov (United States)

    H. T. Odum; George Ann Briscoe; C. B. Briscoe

    1970-01-01

    After relatively high levels of fallout retention were dicovered in the epiphytic mossy forest of the Luquillo Mountains durin 1962, a survey of the distribution of radioactivity in the rain forest system was made with beta counting of 1500 samples supplemented with gamma spectra. High levels, up to 4138 counts per minute per gram, were found mainly in or on green...

  13. Ingestion of Nevada Test Site Fallout: Internal dose estimates

    International Nuclear Information System (INIS)

    Whicker, F.W.; Kirchner, T.B.; Anspaugh, L.R.

    1996-01-01

    This paper summarizes individual and collective dose estimates for the internal organs of hypothetical yet representative residents of selected communities that received measurable fallout from nuclear detonations at the Nevada Test Site. The doses, which resulted from ingestion of local and regional food products contaminated with over 20 radionuclides, were estimated with use of the PATHWAY food-chain-transport model to provide estimates of central tendency and uncertainty. The thyroid gland received much higher doses than other internal organs and tissues. In a avery few cases, infants might have received thyroid doses in excess of 1 Gy, depending on location, diet, and timing of fallout. 131 I was the primary thyroid dose contributor, and fresh milk was the main exposure pathway. With the exception of the thyroid, organ doses from the ingestion pathway were much smaller (<3%) than those from external gamma exposure to deposited fallout. Doses to residents living closest to the Nevada Test Site were contributed mainly by a few fallout events; doses to more distantly located people were generally smaller, but a greater number of events provided measurable contributions. The effectiveness of different fallout events in producing internal organ doses through ingestion varied dramatically with seasonal timing of the test, with maximum dose per unit fallout occurring for early summer depositions when milk cows were on pasture and fresh, local vegetables were used. Within specific communities, internal doses differed by age, sex, and lifestyle. Collective internal dose estimates for specific geographic areas are provided

  14. Radionuclide concentrations in ground level air and precipitation in South Germany from 1976 to 1982

    International Nuclear Information System (INIS)

    Hoetzl, H.; Rosner, G.; Winkler, R.

    1983-08-01

    The activity concentrations of fallout radionuclides from atmospheric nuclear test explosions and of Be-7 in ground level air and precipitation have been determined by the Institut fuer Strahlenschutz at Munich-Neuherberg since 1970. While methods and results from 1970 to 1975 have been published in a previous report, the present report describes the revised program which includes now the naturally occurring nuclides Pb-210 and Po-210, as well as H-3. Sampling methods, analytical techniques and measuring procedures are given. The results up to the end of 1982 are reported and seasonal and long-term variations of radionuclide concentrations as well as frequency distributions of the data are discussed. The data are compared with those of other stations. As a consequence of some recent atmospheric nuclear test explosions by the People's Republic of China also short-lived radionuclides have been detected in ground level air and precipitation. The radiation exposure due to the radioactivity in ground level air and precipitation is estimated. (orig.)

  15. Radioactive fallout over South Africa during 1974-1983

    International Nuclear Information System (INIS)

    Brits, R.J.N.; Van der Bank, D.J.; Moolman, E.W.; Bain, C.A.R.; Van As, D.; Van derwesthuizen, G.S.H.

    1985-05-01

    NUCOR is routinely monitoring air and rainwater for radioactive fallout from atmospheric sources. Air humidity is continuously collected and analysed for tritium. Milk samples are obtained from a number of places throughout the country. These samples are analysed to detect timeously any build-up of radionuclides in soil and plants. Only a few atmosperic nuclear tests have been conducted (by China) since the previous report period of 1965 to 1973. The fallout from these sources over South Africa is extremely small and it is mainly cosmogenic radioactivity, viz 3 H and 7 Be, that is detected

  16. Health effects from fallout.

    Science.gov (United States)

    Gilbert, Ethel S; Land, Charles E; Simon, Steven L

    2002-05-01

    This paper primarily discusses health effects that have resulted from exposures received as a result of above-ground nuclear tests, with emphasis on thyroid disease from exposure to 131I and leukemia and solid cancers from low dose rate external and internal exposure. Results of epidemiological studies of fallout exposures in the Marshall Islands and from the Nevada Test Site are summarized, and studies of persons with exposures similar to those from fallout are briefly reviewed (including patients exposed to 131I for medical reasons and workers exposed externally at low doses and low dose rates). Promising new studies of populations exposed in countries of the former Soviet Union are also discussed and include persons living near the Semipalatinsk Test Site in Kazakhstan, persons exposed as a result of the Chernobyl accident, and persons exposed as a result of operations of the Mayak Nuclear Plant in the Russian Federation. Very preliminary estimates of cancer risks from fallout doses received by the United States population are presented.

  17. Evaluation of 7Be fallout spatial variability

    International Nuclear Information System (INIS)

    Pinto, Victor Meriguetti

    2011-01-01

    The cosmogenic radionuclide beryllium-7 (Be) is produced in the atmosphere by cosmic particle reactions and is being used as a tracer for soil erosion and climatic processes research. After the production, 7 Be bonds to aerosol particles in the atmosphere and is deposited on the soil surface with other radionuclide species by rainfall. Because of the high adsorption on soil particles and its short half-life of 53.2 days, this radionuclide follows of the erosion process and can be used as a tracer to evaluate the sediment transport that occurs during a single rain event or short period of rain events. A key assumption for the erosion evaluation through this radiotracer is the uniformity of the spatial distribution of the 7 Be fallout. The 7 Be method was elaborated recently and due to its few applications, some assumptions related to the method were not yet properly investigated yet, and the hypothesis of 7 Be fallout uniformity needs to be evaluated. The aim of this study was to evaluate the 7 Be fallout spatial distribution through the rain water 7 Be activity analysis of the first five millimeters of single rain events. The rain water was sampled using twelve collectors distributed on an experimental area of about 300 m2 , located in the campus of Sao Paulo University, Piracicaba. The 7 Be activities were measured using a 53% efficiency gamma-ray spectrometer from the Radioisotope laboratory of CENA. The 7 Be activities in rain water varied from 0.26 to 1.81 Sq.L - 1, with the highest values in summer and lowest in spring. In each one of the 5 single events, the spatial variability of 7 Se activity in rain water was high, showing the high randomness of the fallout spatial distribution. A simulation using the 7 Be spatial variability values obtained here and 7 Se average reference inventories taken from the literature was performed determining the lowest detectable erosion rate estimated by 7 Be model. The importance of taking a representative number of samples to

  18. Microcomputer-based systems for automatic control of sample irradiation and chemical analysis of short-lived isotopes

    International Nuclear Information System (INIS)

    Bourret, S.C.

    1974-01-01

    Two systems resulted from the need for the study of the nuclear decay of short-lived radionuclides. Automation was required for better repeatability, speed of chemical separation after irradiation and for protection from the high radiation fields of the samples. A MCS-8 computer was used as the nucleus of the automatic sample irradiation system because the control system required an extensive multiple-sequential circuit. This approach reduced the sequential problem to a computer program. The automatic chemistry control system is a mixture of a fixed and a computer-based programmable control system. The fixed control receives the irradiated liquid sample from the reactor, extracts the liquid and disposes of the used sample container. The programmable control executes the chemistry program that the user has entered through the teletype. (U.S.)

  19. Time-separated oscillatory fields for high-precision mass measurements on short-lived Al and Ca nuclides

    CERN Document Server

    George, Simon; Blank, B.; Blaum, K.; Breitenfeldt, M.; Hager, U.; Herfurth, F.; Herlert, A.; Kellerbauer, A.; Kluge, H.J.; Kretzschmar, M.; Lunney, D.; Savreux, R.; Schwarz, Andreas S.; Schweikhard, L.; Yazidjian, C.

    2008-01-01

    High-precision Penning trap mass measurements on the stable nuclide $^{27}$Al as well as on the short-lived radionuclides $^{26}$Al and $^{38,39}$Ca have been performed by use of radio-frequency excitation with time-separated oscillatory fields, i.e. Ramsey's method, as recently introduced for the excitation of the ion motion in a Penning trap, was applied. A comparison with the conventional method of a single continuous excitation demonstrates its advantage of up to ten times shorter measurements. The new mass values of $^{26,27}$Al clarify conflicting data in this specific mass region. In addition, the resulting mass values of the superallowed $\\beta$-emitter $^{38}$Ca as well as of the groundstate of the $\\beta$-emitter $^{26}$Al$^{m}$ confirm previous measurements and corresponding theoretical corrections of the ft-values.

  20. Results of ten years study of Chernobyl NPP release fallout properties and behaviour in soils

    International Nuclear Information System (INIS)

    Ivanov, Yu.; Kashparov, V.A.; Levchuk, S.; Protsak, V.; Zvaritch, S.; Khomutinin, Yu.; Oreshich, L.

    1997-01-01

    Radioactive contamination of territories of Ukrainian and Byelorussian Polesye as a result of ChNPP accidental release is characterized by high level of un-homogenity of fallout properties (physico-chemical properties, radionuclide composition etc.), density of the territory contamination by long-lived radionuclides. On the other hand, the soil-plant cover of contaminated territory is presented by large set of soils, characterized by contrast physico-chemical and water-physical properties. Peculiarities of the behavior of different radionuclides, represented initially by various components of radioactive fallout, in soils, as a first link of migration chains are considered

  1. Radioactive fallout in air and rain: results to the end of 1976

    International Nuclear Information System (INIS)

    Cambray, R.S.; Fisher, E.M.R.; Eakins, J.D.; Peirson, D.H.

    1977-04-01

    Samples of atmospheric dust and rainwater have been collected from the United Kingdom and elsewhere. Results are presented an analyses of these samples for various fission products and certain other radionuclides. The average concentration of the long-lived fission product caesium-137 in air in the United Kingdom was, in 1976, about one-third of that in 1975 and about 1% of the maximum which was reached in 1963 to 64. The concentration in rain and the deposition of caesium-137 and strontium-90 averaged over the United Kingdom for 1976 were about half those for 1975. No barium-140 or iodine-131, indicative of recent atmospheric tests, was detected in the United Kingdom after the Chinese explosion on 24 January 1976 but measurable concentrations were detected in air at Hong Kong during February. Fresh activity from the Chinese explosion on 26 September 1976 was detected in the United Kingdom. The peak deposition of iodine-131 that occurred in the second week in Octber was greater than at any time since January 1963 although the total deposition of iodine-131 was less than one-tenth of that in 1962 to 63. Trace amounts of fresh activity attributable to the high-yield Chinese explosion of 17 November were detected in the United Kingdom in December 1976. In the southern hemisphere the mean concentration of caesium-137 in air in 1976 was about half that in 1975. An estimate is made of the worldwide deposit of caesium-137 and strontium-90. The gamma and beta-ray dose rates from fallout at Chilton are estimated from the observed deposition. Measurements of short-lived fission products in air and rain are given in an Appendix. (author)

  2. Harvard--MIT research program in short-lived radiopharmaceuticals

    International Nuclear Information System (INIS)

    1991-03-01

    This report describes progress on five projects. The first project showed a 1000 fold concentration of the cationic complex 99m Tc (MIBI) in heart cell mitochondria vs heart cell cytoplasm, as determined by high resolution electron probe microanalysis. Additional technetium-99m based complexes are being developed and tested. The second project involves evaluating technetium acetylacteonates as potential indicators of cerebral blood flow. An intermediate in the synthesis of a technetium porphyrin complex has been synthesized; an oxotechnetium(V)-2,4-pentanedione complex has been prepared and is currently being characterized. The third project involves using radio labelled antibodies for diagnosis and treatment of cancer. An early discovery was that chloramine-T based iodination protocols resulted in a reversal of the charge on mouse lgGs. Immunoperoxidase-labelled monoclonal antibody MOv 18 was shown to bind specifically to the most frequent ovarian aderon carcinomas, and not to healthy tissue, making this antibody a good candidate for immunotherapy or immunodetection. Work on a specific immunotherapy protocol suffered a setback when one reagent, a 125 I-biotin complex, proved to be unstable in vivo. The fourth project involves labelling antibodies with positron emitting radionuclides. Radiofluorination was accomplished through reductive alkylation of 18 F-aldehyde, or pentafluorophenyl esters. Radioiodination was accomplished using alkyl-tin derivation exchange. The fifth project examined antibody modification for use in radioimmune imaging. Technetium-99m-labelled lgG was shown to be biologically equivalent to Indium-III-labelled lgG for imaging focal sites of inflamation. Also, Indium III labelling of small bioactive peptides was examined as a means of imaging important physiological processes. 44 refs., 2 figs

  3. Nuclear fallout shelter

    International Nuclear Information System (INIS)

    Elton, J.

    1982-01-01

    A nuclear fallout shelter, to be buried below ground level exposing only an access hatch with a cover and ventilators, is constructed of two preformed hollow end sections connected by one or more preformed hollow tubular intermediate sections. The ventilators include a filter for removing radioactive particles from the air entering the shelter. The sections may be moulded shells of glass fibre reinforced plastics material having inwardly directed peripheral end flanges to enable the sections to be bolted together from inside the shelter after they have been positioned in an excavated trench. (author)

  4. Radionuclide ratios in wet and dry deposition samples from June 1976 through December 1977

    International Nuclear Information System (INIS)

    Gavini, M.B.

    1978-01-01

    238 Pu, 239 Pu and 137 Cs in rain and dry fallout and 90 Sr in rain samples were measured at Woods Hole, Massachusetts, from June 1976 through December 1977. The dry fallout was estimated to be about 7.8% of the total deposition of 239 Pu and 137 Cs. 239 Pu/ 137 Cs ratios, almost constant at about 0.011 in rain or dry fallout, February through December 1977, suggested that fractionation between the refractory and volatile radionuclides is insignificant in stratospheric fallout. This supports the idea of regional homogeneity of radionuclide ratios in fallout. (Auth.)

  5. Historical review of short-lived isotope applications in New Zealand

    International Nuclear Information System (INIS)

    More, R.D.

    1986-01-01

    Production of short-lived isotopes, nitrogen 13, fluorine 18 and carbon 11 with a small Van de Graaff accelerator. Applications of these isotopes in uptake and photosynthetic translocation studies in plants, and fluorine tracing in dental studies

  6. Fallout Deposition in the Marshall Islands from Bikini and Enewetak Nuclear Weapons Tests

    OpenAIRE

    Beck, Harold L.; Bouville, André; Moroz, Brian E.; Simon, Steven L.

    2010-01-01

    Deposition densities (Bq m-2) of all important dose-contributing radionuclides occurring in nuclear weapons testing fallout from tests conducted at Bikini and Enewetak Atolls (1946-1958) have been estimated on a test-specific basis for all the 31 atolls and separate reef islands of the Marshall Islands. A complete review of various historical and contemporary data, as well as meteorological analysis, was used to make judgments regarding which tests deposited fallout in the Marshall Islands an...

  7. Fallout Concentration Various Environmental Samples in Indonesia

    International Nuclear Information System (INIS)

    Sutarman

    2001-01-01

    The testing of nuclear weapons have been carried out by the advanced countries, such as United States, Russian Federation, United Kingdom, France, China, India and Pakistan, since about 1945 until 1998. Nuclear weapons tests were conducted at various locations, on and above the earth's surface or underground or on and under the ocean's surface. Nuclear explosions caused the radionuclides of fission product, such as 131 l, 89 Sr, 90 Sr, 134 Cs, 137 Cs, and 239 Pu released to the atmospheric layer. In the atmospheric layer, the long-lived radionuclides, i.e, 90 Sr dan 137 Cs will be distributed into the environment as the fallout radionuclides, and deposited in the various environmental samples (soil, water, and biota). In general, at several locations in Indonesia the 90 Sr and 137 Cs in the various environmental samples still can be detected. The data of measurement results of 90 Sr and 137 Cs concentrations were generally lower than that from some countries in the northern hemisphere. (author)

  8. Strontium 90 fallout prediction

    International Nuclear Information System (INIS)

    Sarmiento, J.L.; Gwinn, E.

    1986-01-01

    An empirical formula is developed for predicting monthly sea level strontium 90 fallout (F) in the northern hemisphere as a function of time (t), precipitation rate (P), latitude (phi), longitude (lambda), and the sea level concentration of stronium 90 in air (C): F(lambda, phi, t) = C(t, phi)[v /sub d/(phi) + v/sub w/(lambda, phi, t)], where v/sub w/(lambda, phi, t) = a(phi)[P(lambda, phi, t)/P/sub o/]/sup b//sup (//sup phi//sup )/ is the wet removal, v/sub d/(phi) is the dry removal and P 0 is 1 cm/month. The constants v/sub d/, a, and b are determined as functions of latitude by fitting land based observations. The concentration of 90 Sr in air is calculated as a function of the deseasonalized concentration at a reference latitude (C-bar/sub r//sub e//sub f/), the ratio of the observations at the latitude of interest to the reference latitude (R), and a function representing the seasonal trend in the air concentration (1 + g): C-bar(t, phi) = C/sub r//sub e//sub f/(t)R(phi)[1 + g(m, phi)]; m is the month. Zonal trends in C are shown to be relatively small. This formula can be used in conjuction with precipitation observations and/or estimates to predict fallout in the northern hemisphere for any month in the years 1954 to 1974. Error estimates are given; they do not include uncertainty due to errors in precipitation data

  9. Measurements of atmospheric fallout in Argentina

    International Nuclear Information System (INIS)

    Canoba, A.C.; Lopez, F.O.; Bruno, H.A.

    1998-01-01

    With the purpose of studying the radioactive fallout present in Argentina from atmospheric nuclear explosions tests that have been conducted recently, an environmental monitoring program, outside the influence of nuclear facilities of Argentina, was undertaken during 1996 and 1997. The levels of Cs-137 and Sr-90 were analysed in samples of air, deposited material (rainwater), milk, an average meal of a standard man and food. During this period, a total of 630 radiochemical analysis were performed on 325 samples of the different matrices described. The concentration levels of the radionuclides analysed in the different environmental matrices are presented and are compared with the values obtained in the environmental monitoring program done during the period 1960-1981. (author) [es

  10. Fallout model for system studies

    International Nuclear Information System (INIS)

    Harvey, T.F.; Serduke, F.J.D.

    1979-01-01

    A versatile fallout model was developed to assess complex civil defense and military effect issues. Large technical and scenario uncertainties require a fast, adaptable, time-dependent model to obtain technically defensible fallout results in complex demographic scenarios. The KDFOC2 capability, coupled with other data bases, provides the essential tools to consider tradeoffs between various plans and features in different nuclear scenarios and estimate the technical uncertainties in the predictions. All available data were used to validate the model. In many ways, the capability is unmatched in its ability to predict fallout hazards to a society

  11. RETROSPECTIVE RECONSTRUCTION OF INTEGRAL IODINE-131 FALLOUT FOR THE SETTLEMENTS OF THE BRYANSK REGION OF RUSSIA ON THE BASIS OF RESULTS OF IODINE-129 CONTENT IN THE SOIL DETERMINATION IN 2008

    Directory of Open Access Journals (Sweden)

    Yu. I. Gavrilin

    2009-01-01

    Full Text Available The article briefly describes the procedure of reconstruction of integral iodine-131 fallouts using fragmentary data on iodine-131 fallouts in May-June 1986, as well as results of determination (in the late period after the accident of iodine-129 concentration in the soil and values of integral fallouts of cesium-137 in the settlements of the Bryansk region of Russia. Results of estimation of integral iodine-131 fallouts (in the area of 32 soil sampling points are presented in the table form. Regularities of ratio (131I/137CsII change in the integral radionuclide fallouts are being determined and values of integral iodine-131 fallouts are being estimatedfor the other settlements of the region with the known values of integral cesium-137 fallouts. It is shown that variability of the average for settlements values of integral iodine-131 fallouts is 70 times less then variability of corresponding integral cesium-137 fallouts.

  12. The real hazards of nuclear fallout

    International Nuclear Information System (INIS)

    Knox, J.B.; Shapiro, C.S.

    1986-01-01

    The paper discusses an article by Carl Sagan entitled ''On minimizing the consequences of nuclear war'' [Nature 317 485 Oct 1985], in the light of the authors' own work on global fallout. Consequences of local fallout, human impact of local fallout, and global fallout calculations using computer models, are all described. (U.K.)

  13. Vehicle emissions of short-lived and long-lived climate forcers: trends and tradeoffs.

    Science.gov (United States)

    Edwards, Morgan R; Klemun, Magdalena M; Kim, Hyung Chul; Wallington, Timothy J; Winkler, Sandra L; Tamor, Michael A; Trancik, Jessika E

    2017-08-24

    Evaluating technology options to mitigate the climate impacts of road transportation can be challenging, particularly when they involve a tradeoff between long-lived emissions (e.g., carbon dioxide) and short-lived emissions (e.g., methane or black carbon). Here we present trends in short- and long-lived emissions for light- and heavy-duty transport globally and in the U.S., EU, and China over the period 2000-2030, and we discuss past and future changes to vehicle technologies to reduce these emissions. We model the tradeoffs between short- and long-lived emission reductions across a range of technology options, life cycle emission intensities, and equivalency metrics. While short-lived vehicle emissions have decreased globally over the past two decades, significant reductions in CO 2 will be required by mid-century to meet climate change mitigation targets. This is true regardless of the time horizon used to compare long- and short-lived emissions. The short-lived emission intensities of some low-CO 2 technologies are higher than others, and thus their suitability for meeting climate targets depends sensitively on the evaluation time horizon. Other technologies offer low intensities of both short-lived emissions and CO 2 .

  14. Radionuclide content of soils from Barrio Islote, Arecibo, Puerto Rico

    International Nuclear Information System (INIS)

    Block, A.McB.; Clements, R.G.

    1976-06-01

    The purpose of this report is to present and interpret gamma ray energy spectra from natural radioactivity and fallout radionuclides measured on soil samples collected in the projected thermonuclear power plant exclusion zone in Barrio Islote, Puerto Rico

  15. Quantifying the contributions of sediment, sediment-P and fertiliser-P from forested, cultivated and pasture areas at the landuse and catchment scale using fallout radionuclides and geochemistry

    International Nuclear Information System (INIS)

    Wallbrink, P.J.; Martin, C.E.; Wilson, C.J.

    2003-01-01

    In this paper we use a combination of fallout nuclides and geochemistry to determine the contributions of sediment and sediment bound phosphorus (sed-P) from the major diffuse sources in the Bundella Creek catchment (8700 ha), NSW, Australia. Sources include surface erosion from cultivated, pasture and steep forested land as well as subsoil erosion from channels and gullies. We determine these contributions to the <10 μm fraction of deposited sediments. Concentrations of P were higher in the surface soils of each landuse than the underlying subsoils, and erosion from these contributed more to offsite sediment-P (∼60%) than did subsoil erosion at the individual landuse scale. At the catchment outlet, the amount of surface sediment eroded from cultivated lands was a factor of ∼84 higher than from pastures; the steep forested lands contributed ∼9 times more than pastures. Sed-P eroded from cultivated land was ∼42 times higher than from pasturelands; the forests were ∼8 times greater than from pastures. At the catchment outlet the largest contribution of sediment (∼70%) and sed-P (∼62%) was from subsoil erosion of gullies and channels within and between the different landuse areas. There was little contribution of sediment or sed-P at the catchment scale from surface erosion of pastures. Concentrations of P were highest in 'storm event' suspended sediment samples taken from the pasture and cultivated areas without gullies. In a suite of samples selected for their high P contents, fertiliser P was detected in two storm event suspended sediment samples and one deposited sediment sample, using the ratio of Nd/P. This suggests fertiliser P may be transported-off land surfaces with sediments and contribute to offsite sediment-P concentrations in some situations. However, the fertiliser contributions were episodic and variable; and probably influenced by particle size selectivity as well as timing of fertiliser application with respect to size and occurrence

  16. Marine biogeochemistry of radionuclides

    International Nuclear Information System (INIS)

    Fowler, S.W.

    1997-01-01

    Radionuclides entering the ocean from runoff, fallout, or deliberate release rapidly become involved in marine biogeochemical cycles. Sources, sinks and transport of radionuclides and analogue elements are discussed with emphasis placed on how these elements interact with marine organisms. Water, food and sediments are the source terms from which marine biota acquire radionuclides. Uptake from water occurs by surface adsorption, absorption across body surfaces, or a combination of both. Radionuclides ingested with food are either assimilated into tissue or excreted. The relative importance of the food and water pathway in uptake varies with the radionuclide and the conditions under which exposure occurs. Evidence suggests that, compared to the water and food pathways, bioavailability of sediment-bound radionuclides is low. Bioaccumulation processes are controlled by many environmental and intrinsic factors including exposure time, physical-chemical form of the radionuclide, salinity, temperature, competitive effects with other elements, organism size, physiology, life cycle and feeding habits. Once accumulated, radionuclides are transported actively by vertical and horizontal movements of organisms and passively by release of biogenic products, e.g., soluble excreta, feces, molts and eggs. Through feeding activities, particles containing radionuclides are ''packaged'' into larger aggregates which are redistributed upon release. Most radionuclides are not irreversibly bound to such particles but are remineralized as they sink and/or decompose. In the pelagic zones, sinking aggregates can further scavenge particle-reactive elements thus removing them from the surface layers and transporting them to depth. Evidence from both radiotracer experiments and in situ sediment trap studies is presented which illustrates the importance of biological scavenging in controlling the distribution of radionuclides in the water column. (author)

  17. A technique for the measurement of electron attachment to short-lived excited species

    International Nuclear Information System (INIS)

    Christophorou, L.G.; Pinnaduwage, L.A.; Bitouni, A.P.

    1990-01-01

    A technique is described for the measurement of electron attachment to short-lived (approx-lt 10 -9 s) excited species. Preliminary results are presented for photoenhanced electron attachment to short-lived electronically-excited states of triethylamine molecules produced by laser two-photon excitation. The attachment cross sections for these excited states are estimated to be >10 -11 cm 2 and are ∼10 7 larger compared to those for the unexcited (ground-state) molecules. 8 refs., 4 figs

  18. New radionuclide generator systems for use in nuclear medicine

    International Nuclear Information System (INIS)

    Atcher, R.W.

    1979-01-01

    A current emphasis in nuclear medicine is to better match the physical lifetime of the radionuclides used in vivo for diagnosis and treatment to the biological lifetime of the diagnostic procedure or to minimize radiation dose to areas other than those to be treated. In many cases the biological lifetime is on the order of minutes. Since the direct production of radionuclides with half lives of minutes requires the user to be near a suitable reactor or accelerator, this study was undertaken to produce short-lived radionuclides indirectly. If a long-lived radionuclide decays into a short-lived radionuclide, quick separation of the daughter activity from the parent enables the user to have a short-lived daughter while freeing him from the constraint of proximity to a cyclotron. Systems where a short-lived daughter is separated from a long-lived parent are called radionuclide generators. Two generator systems were developed for use in nuclear medicine, one in diagnostic work and the other for therapeutic work. The yield and breakthrough characteristics were within the limits required to minimize unnecessary radiation exposure in patients. Two parent radionuclides were produced using 4 He beams available from medium energy cyclotrons. The yield was high enough to produce generators that would be useful in clinical applications

  19. Local fall-out and the animal food chain

    International Nuclear Information System (INIS)

    Prat, G.; Mercier, F.J.

    1967-01-01

    The local consequences of fresh fall-out, especially in the case of atmospheric nuclear explosions, are reviewed from the point of view of the internal contamination of the consumer of foodstuffs of animal origin. The edibility of foodstuffs derived from animals having grazed in the presence of fall-out is evaluated both from the wholesome and radio-toxicological points of view. The contamination level of these foodstuffs is calculated as a function of the ground fall-out, and of agronomical and ecological parameters for each radio-nuclide of the animal food chain. The internal exposure of the human consumer is calculated from this level as a function of the diet and of various parameters especially temporal. The equivalent dose to each critical organ, including the digestive tract is deduced from the burdens of each organ. From this a nutritional hygiene in the areas affected by fall-out is obtained, in relationship to the action levels fixed by the responsible authorities in exceptional circumstances. Criteria for these action levels are given as function of the food rations. (authors) [fr

  20. Radionuclide composition in the surface layer of particles in the troposphere and stratosphere falls

    International Nuclear Information System (INIS)

    Prokof'ev, O.N.

    1977-01-01

    Radionuclide content in troposphere and stratosphere fall-outs as well as radionuclide washing-off from fall-out particle; are important to determine internal irradiation doses received by separate critical organs of human body. In surface-contaminated products (floury products of grain contaminated while in ears, vegetables, fruits, berries, noncovered or insufficiently covered products during fall-outs) radionuclides initially (in an initial state) are connected with fall-out particles. Radionuclides in biologically contaminated products (milk, meat etc.) are not connected with the particles and have the assimilable form. However, the degree of radionuclide transition from forage (grasses, hay etc.) surface-contaminated as a results of fall-outs into animal produce (milk, meat etc.) also depends on radionuclide washing-off from fall-out particles, which in the latter results from the formation nature and a kind of particles of the main substance. Radionuclide washing-off degree (and, consequently, biological availability) by glazed silicate particles is caused by radionuclide distribution between particle volume and surface in an appropriate sample. According to Israel Yu.A. method calculated were the shares of surface-bound atoms for all the particle totality in an explosion cloud for mass chains, which composition includes biologically important radionuclides. Particle solidification time is taken to equal 7 and 40s. Independent yields of chain radionuclides and its total yield are taken for 228 U fission under 14 MeV neutron effect. The calculation results are presented in the tables

  1. Radioactive fallout in food and agriculture

    International Nuclear Information System (INIS)

    Winteringham, F.P.W.

    1989-01-01

    Part 1 of this review is designed to provide an up-dated background to the subject in relation to FAO's interests and responsibilities in scientifically accurate but non-technical language. Part 2 is concerned more specifically with the problems of radioactive fallout over pasture and cultivated soils. Moreover, it is mainly concerned with problems of international significance under peacetime conditions and which are likely only to arise as a result of a major nuclear reactor accident, or, possibly, some unintended nuclear explosion. However, relatively local problems of soil contamination could arise as a result of other kinds of accident. In the report the natural occurrence of radionuclides, and radiation exposure as a fact of life in the human environment, are indicated. Exposure to ionizing radiation from natural and man-made sources are compared. The behaviour and significance of radionuclides in ecosystems are briefly illustrated. Land-based nuclear powr stations and nuclear-powered ships and submarines are identified as the major potential accident hazards to agriculture or fisheries under peacetime conditions. 216 refs, figs and tabs

  2. A new integrative methodology for desertification studies based on magnetic and short-lived radioisotope measurements

    International Nuclear Information System (INIS)

    Oldfield, F.; Higgitt, S.R.; Maher, B.A.; Appleby, P.G.; Scoullos, M.

    1986-01-01

    The use of mineral magnetic measurements and short-lived radioisotope studies with 210 Pb and 137 Cs is discussed within the ecosystem watershed conceptual framework. Used in conjunction with geomorphological, sedimentological, palaeoecological and geochemical techniques, these methods can form the core of an integrated multidisciplinary study of desertification and erosion processes on all relevant temporal and spatial scales. 30 refs.; 4 figs

  3. Applications of short-lived isotopes in agricultural research in New Zealand

    International Nuclear Information System (INIS)

    McCallum, G.J.; More, R.D.; McNaughton, G.S.; Minchin, P.E.H.; Presland, M.R.; Stout, J.D.

    1981-01-01

    The use of the short-lived isotopes 11 C and 13 N in agricultural research studies in New Zealand is reviewed. The methods employed to produce these radioisotopes using a 3 MV Van de Graaff accelerator are given. Experiments on transport processes and the uptake of nutrient by plants, and the study of soil processes are described. (Auth.)

  4. Analysing environmental and fishing effects on a short-lived species ...

    African Journals Online (AJOL)

    Short-lived species are extremely dependent on the seasonal and interannual variability of environmental conditions, and determining their stock status is often difficult. This study investigates the effects of environmental variability and fishing pressure on the stock of octopus Octopus vulgaris in Senegalese waters over a ...

  5. Disentangling the effects of CO2 and short-lived climate forcer mitigation

    NARCIS (Netherlands)

    Rogelj, J.; Schaeffer, M.; Meinshausen, M.; Shindell, D.T.; Hare, W.; Klimont, Z.; Velders, G.J.M.; Amann, M.; Schellnhuber, H.J.

    2014-01-01

    Anthropogenic global warming is driven by emissions of a wide variety of radiative forcers ranging from very short-lived climate forcers (SLCFs), like black carbon, to very long-lived, like CO2. These species are often released from common sources and are therefore intricately linked. However, for

  6. Short Lived Fission Product Yield Measurements in 235U, 238U and 239Pu

    Science.gov (United States)

    Silano, Jack; Tonchev, Anton; Tornow, Werner; Krishichayan, Fnu; Finch, Sean; Gooden, Matthew; Wilhelmy, Jerry

    2017-09-01

    Yields of short lived fission products (FPYs) with half lives of a few minutes to an hour contain a wealth of information about the fission process. Knowledge of short lived FPYs would contribute to existing data on longer lived FPY mass and charge distributions. Of particular interest are the relative yields between the ground states and isomeric states of FPYs since these isomeric ratios can be used to determine the angular momentum of the fragments. Over the past five years, a LLNL-TUNL-LANL collaboration has made precision measurements of FPYs from quasi-monoenergetic neutron induced fission of 235U, 238U and 239Pu. These efforts focused on longer lived FPYs, using a well characterized dual fission chamber and several days of neutron beam exposure. For the first time, this established technique will be applied to measuring short lived FPYs, with half lives of minutes to less than an hour. A feasibility study will be performed using irradiation times of < 1 hour, improving the sensitivity to short lived FPYs by limiting the buildup of long lived isotopes. Results from this exploratory study will be presented, and the implications for isomeric ratio measurements will be discussed. This work was performed under the auspices of US DOE by LLNL under Contract DE-AC52-07NA27344.

  7. Short-lived brain state after cued motor imagery in naive subjects

    NARCIS (Netherlands)

    Pfurtscheller, G.; Scherer, R.; Müller-Putz, G.R.; Lopes da Silva, F.H.

    2008-01-01

    Multi-channel electroencephalography recordings have shown that a visual cue, indicating right hand, left hand or foot motor imagery, can induce a short-lived brain state in the order of about 500 ms. In the present study, 10 able-bodied subjects without any motor imagery experience (naive subjects)

  8. The development of fast tantalum foil targets for short-lived isotopes

    CERN Document Server

    Bennett, J R J; Drumm, P V; Ravn, H L

    2003-01-01

    The development of fast tantalum foil targets for short-lived isotopes was discussed. It was found that the effusion was faster but the diffusion out of the foils was a limiting factor. The performance of the targets at ISOLDE with beams of **1**1Li, **1**2Be and **1**4Be was also analyzed. (Edited abstract) 13 Refs.

  9. Transport and deposition of nano-particles. Application to the free action of short-lived radon daughters

    International Nuclear Information System (INIS)

    Malet, J.

    1997-01-01

    Short-lived radon daughters ( 218 Po, 214 Pb, 214 Bi, and 214 Po) are important contributors to the natural average annual individual dose. The models describing the evolution of these aerosol in a house depend critically on a parameter, the 218 Po deposition velocity, which, although aerosol deposition has been extensively studied, is poorly known. A numerical and experimental study is thus carried out for a simple case: deposition in a cylindrical tube under laminar flow condition. The numerical results help understanding the difference between the transport and deposition of these radionuclides and those of non radioactive aerosols. Comparison of these well environment does not give satisfactory correlation, requiring the study of phenomena that may affect deposition. The first of these is the possible variation in the e 218 Po diffusion coefficient. Furthermore, experiments coupled with numerical calculations show that this variation could be due to 218 Po neutralization. The second phenomenon concerns the effect of the surface type, which is also shown experimentally. By modelling the neutralization and using results with a piratically smooth surface, good numerical/experimental correlations are obtained. Understanding this simple case than makes possible studying a more complex case: deposition in controlled turbulent flow. Two theories are thus experimentally validated. In addition, a 218 Po deposition velocity representative of our experimental conditions is determined. Finally, we report a feasibility study of radon daughters transport and deposition in a ventilated chamber taking into account all the involved phenomena. (author)

  10. Measurement method of activation cross-sections of reactions producing short-lived nuclei with 14 MeV neutrons

    CERN Document Server

    Kawade, K; Kasugai, Y; Shibata, M; Iida, T; Takahashi, A; Fukahori, T

    2003-01-01

    We describe a method for obtaining reliable activation cross-sections in the neutron energy range between 13.4 and 14.9 MeV for the reactions producing short-lived nuclei with half-lives between 0.5 and 30 min. We noted neutron irradiation fields and measured induced activities, including (1) the contribution of scattered low-energy neutrons, (2) the fluctuation of the neutron fluence rate during the irradiation, (3) the true coincidence sum effect, (4) the random coincidence sum effect, (5) the deviation in the measuring position due to finite sample thickness, (6) the self-absorption of the gamma-ray in the sample material and (7) the interference reactions producing the same radionuclides or the ones emitting the gamma-ray with the same energy of interest. The cross-sections can be obtained within a total error of 3.6%, when good counting statistics are achieved, including an error of 3.0% for the standard cross-section of sup 2 sup 7 Al (n, alpha) sup 2 sup 4 Na. We propose here simple methods for measuri...

  11. A general approach to transform a lake model for one radionuclide (radiocesium) to another (radiostrontium) and critical model tests using data for four Ural lakes contaminated by the fallout from the Kyshtym accident in 1957

    Energy Technology Data Exchange (ETDEWEB)

    Haakanson, Lars E-mail: lars.hakanson@natgeog.uu.se; Sazykina, Tatiana G.; Kryshev, Ivan I

    2002-07-01

    This paper presents results of a model test carried out within the framework of the COMETES project (EU). The aim of the work was to change the structure of the MOIRA lake model for radiocesium so that it can be applied more generally for, in principle, all types of radionuclides and heavy metals. This general lake model is used within the MOIRA decision support system (DSS; MOIRA and COMETES are acronyms for EU-projects). The model is based on a set of differential equations and a specific modelling structure. It incorporates all important fluxes to, from and within lakes in a general manner. Yet the model is driven by a minimum of variables accessible from standard maps and monitoring programs. The model can be separated into two parts, a general part with equations applicable for all types of water pollutants and a substance-specific part. This model has previously been validated for {sup 137}Cs from many lakes covering a wide domain and yielded excellent predictive power. The alterations discussed in this work are meant to be general and radiostrontium is used as a typical element. Radiostrontium is known to be more mobile than radiocesium and all abiotic parts of the model handling fixation and mobility have been altered. The new model for {sup 90}Sr has been critically tested using data from four lakes heavily contaminated with {sup 90}Sr from the Kyshtym accident in the Southern Urals, Russia, using empirical data from a period from 1958 to 1995 for {sup 90}Sr in fish (here goldfish), water and sediments.

  12. Modelling the external radiation exposure from the Chernobyl fallout using data from the Swedish municipality measurement system.

    Science.gov (United States)

    Jönsson, Mattias; Tondel, Martin; Isaksson, Mats; Finck, Robert; Wålinder, Robert; Mamour, Afrah; Rääf, Christopher

    2017-11-01

    In connection with the Chernobyl fallout and the subsequent deposition of radionuclides in Sweden, Swedish municipalities launched a measurement program to monitor the external radiation exposure. This program encompasses measurements of the ambient dose equivalent rate 1 m above ground at selected locations, and repeats those measurements at the same locations at 7-month intervals. Measurement data compiled from the seven locations with the highest deposition were combined with data from aerial surveys since May 1986 of ground deposition of 137 Cs, high-resolution gamma spectrometry performed at four locations in May 1986, and measurements from fixed continuous air gamma rate monitoring stations from 28 April to 15 May 1986. Based on these datasets, a model of the time pattern of the external dose rate in terms of ambient dose equivalent rate from the Chernobyl fallout was developed. The decrease in the ambient dose equivalent rate could, on average, be described by a four-component exponential decay function with effective half-times of 6.8 ± 0.3 d, 104 ± 26 d, 1.0 ± 0.02 y and 5.5 ± 0.09 y, respectively. The predominant contributions to the external dose rate in the first month were from short-lived fission products superseded by 134 Cs and then 137 Cs. Integrated over 70 y and using extrapolation of the curve fits, our model predicts that 137 Cs contributes about 60% and 134 Cs contributes about 30% of the external effective dose at these seven locations. The projected time-integrated 70 y external effective dose to an unshielded person from all nuclides per unit total activity deposition of 137 Cs is estimated to be 0.29 ± 0.0.08 mSv/(kBq m -2 ). These results are in agreement with those found in Chernobyl contaminated Russian forest areas, and emphasize the usefulness of maintaining a long-term and regular measurement program in contaminated areas. Copyright © 2017 Elsevier Ltd. All rights reserved.

  13. Gamma ray spectra recorded from the fallout collected in May 1986

    International Nuclear Information System (INIS)

    Cristu, M.I.

    1987-07-01

    An analysis of the gamma ray spectra recorded from the fallout collective in Bucharest and Brasov in May, 1986 was carried out. Relative activities of the assigned radionuclides were computed and the duration of the 235 U fuel irradiation has been deduced. (author)

  14. Public health impact of fallout from British nuclear weapons tests in Australia, 1952-1957

    International Nuclear Information System (INIS)

    Wise, K.N.; Moroney, J.R.

    1992-05-01

    During the period 1952-1957, Britain conducted 12 full-scale nuclear weapons tests in Australia in five series, viz. Hurricane(1952), Totem(1953), Mosaic(1956), Buffalo(1956) and Antler(1957). Radioactive fallout from the tests reached many parts of Australia. This report reviews the pathways by which the radionuclides in the fallout could have irradiated the population. The methodology is presented for estimating the radiation doses and values are derived from the available data. The possible effect that the radiation exposure had on public health is assessed. Estimation of the radiation doses is approached in two parts: (a) the contributions from the Mosaic, Buffalo and Antler series which were monitored, and (b) the contributions from the Hurricane and Totem series for which there are few fallout data. In part (a), the activities of the radionuclides making up the measured fallout are established by calculation. Standard models are then used to derive the radiation doses for the population centres - from external radiation, from ingestion of radionuclides in food and from inhalation of radionuclides in air. A simple treatment is adopted to estimate radiation doses from drinking contaminated water. For Part (b), the data assembled in (a) provide the basis for developing statistical models for predicting radiation doses from weapon yields and trajectories of the radioactive clouds. The models are then applied to give the radiation doses to population centres following the tests in Hurricane and Totem, using their yields and trajectories. 71 refs., 20 tabs., 8 figs

  15. Utilization of cesium-137 environmental contamination from fallout in erosion and sedimentation studies

    International Nuclear Information System (INIS)

    Guimaraes, M.F. da; Pessenda, L.C.R.; Fernandes, E.A.N.; Freire, O.; Nascimento Filho, V.F. do; Ferraz, E.S.B.

    1988-01-01

    The radioactivity of cesium-137 from fallout in different soils profiles for erosion and sedimentation studies are described. The potential of this technique for hydrographic basin in Piracicaba/Sao Paulo is evaluated. Due to the existence of natural radionuclides in soil, with energy near to cesium-137, the soil samples are determined by a high-purity Ge detectors. (author)

  16. Plutonium fallout at Fayetteville, AR

    International Nuclear Information System (INIS)

    Sandoval, D.N.; Essien, I.O.; Kuroda, P.K.

    1985-01-01

    It is well established that atmospheric Pu fallout has its origin in the testing of nuclear devices and satellite accidents. Monitoring injections of Pu during the testing of nuclear devices can be useful in characterizing the detonation and subsequently tagging its global fallout. Since Pu uptake pathway into humans is mainly through the respiratory and digestive systems, it is important to know about the behavior of Pu in the atmosphere. Snow and rain samples were collected between Jan 1981 and April 1983, and analyzed for plutonium

  17. Losses of Sr/sup 90/, Sr/sup 89/, and I/sup 131/ from fallout-contaminated plants

    Energy Technology Data Exchange (ETDEWEB)

    Martin, W E

    1964-11-01

    During the early period following local fallout, and during periods of maximal worldwide fallout, the entry of radionuclides into terrestrial food-chains is due primarily to the external contamination of plants and secondarily to the uptake of radionuclides from contaminated soil. Studies were undertaken to estimate the rates of radionuclide loss from fallout-contaminated vegetation and hence from the diets of herbivores living in a fallout field. On the fifth, fifteenth, thirtieth, and sixtieth days after an underground nuclear explosion (Operation Sedan) at the Nevada Test Site, plant samples were collected from twenty representative locations in the fallout field and analyzed to determined the concentrations (pc/g dry wt) of /sup 90/Sr, /sup 89/Sr, and /sup 131/I at the times of collections. While the radioactive half lives of /sup 90/Sr, /sup 89/Sr, and /sup 131/I are approximately 27.7 years, 53 days, and 8.04 days respectively, their average effective half-lives on fallout-contaminated plants, during the period from 5 to 30 days after the detonation, were 27.8 days, 17.8 days, and 5.0 days respectively. Losses of /sup 90/Sr were attributed to radioactive decay and to the removal of fallout particles and foliage by wind and/or other mechanical disturbances. Losses of /sup 90/Sr and /sup 89/Sr were attributed to radioactive decay and to the removal of fallout particles and foliage by wind and/or other mechanical disturbances. Losses of /sup 131/I were attributed to radioactive decay, to mechanical disturbance, and to the vaporization of /sup 131/I from the fallout particles retained on foliage.

  18. Neutron-induced cross sections of short-lived nuclei via the surrogate reaction method

    Directory of Open Access Journals (Sweden)

    Morel P.

    2011-10-01

    Full Text Available The measurement of neutron-induced cross sections of short-lived nuclei is extremely difficult due to the radioactivity of the samples. The surrogate reaction method is an indirect way of determining cross sections for nuclear reactions that proceed through a compound nucleus. This method presents the advantage that the target material can be stable or less radioactive than the material required for a neutron-induced measurement. We have successfully used the surrogate reaction method to extract neutron-induced fission cross sections of various short-lived actinides. In this work, we investigate whether this technique can be used to determine neutron-induced capture cross sections in the rare-earth region.

  19. Neutron-induced cross sections of short-lived nuclei via the surrogate reaction method

    Directory of Open Access Journals (Sweden)

    Tassan-Got L.

    2012-02-01

    Full Text Available The measurement of neutron-induced cross sections of short-lived nuclei is extremely difficult due to the radioactivity of the samples. The surrogate reaction method is an indirect way of determining cross sections for nuclear reactions that proceed through a compound nucleus. This method presents the advantage that the target material can be stable or less radioactive than the material required for a neutron-induced measurement. We have successfully used the surrogate reaction method to extract neutron-induced fission cross sections of various short-lived actinides. In this work, we investigate whether this technique can be used to determine neutron-induced capture cross sections in the rare-earth region.

  20. Determination of short-lived trace elements in environmental samples by neutron activation analysis

    International Nuclear Information System (INIS)

    Wardani, S.; Sihombing, E.; Hamzah, A.; Rochidi; Hery, P.S.; Hartaman, S.; Iman, J.

    1998-01-01

    Concentration of a short-lived trace elements in environmental samples were determined by neutron activation analysis, a counting loss often occur due to the high counting rate. A Pile-Up Rejecter (PUR) electric circuit was installed in counting a short-lived trace elements by a γ-ray spectrometer in order to correct a counting loss. The samples were irradiated for 30∼60 seconds at neutron flux of 3.5 x 10 12 n.cm -2 .s -1 , then the samples cooled for 120 second and counted for 180 second using this system. The nuclides concentration in the varieties environmental samples have a difference analysis result, was more accurate and precise, which the measured result would be 30 % more higher by PUR system than the result would be counted using a conventional γ-ray spectrometry method

  1. Studies on short-lived fission products at the Mainz TRIGA reactor

    International Nuclear Information System (INIS)

    Trautmann, N.

    1974-01-01

    Neutron-rich nuclei of medium mass number are produced by thermal-neutron-induced fission of heavy elements, e.g., 235 U, 239 Pu, and 249 Cf. Pulse irradiations lead to an enhancement of the ratio of short-lived activities to the accompanying longer-lived components. One approach for investigating the properties of short-lived nuclei consists in a combination of rapid chemical separations with higher-resolution gamma spectroscopy. This is demonstrated by the isolation of neutron-rich isotopes of niobium by sorption on glass and of ruthenium by solvent extraction. Other rapid separation procedures from aqueous solutions are briefly summarized and a few examples for their application in nuclear fission- and delayed neutron studies are given. Some experiments with an on-line mass separator of the ISOLDE-type, using chemical targets, are described. (U.S.)

  2. Aube storage centre for short-lived low- and intermediate-level wastes. Annual report 2009

    International Nuclear Information System (INIS)

    2010-06-01

    The National Radioactive Waste Management Agency (Andra), was established by the December 1991 Waste Act as a public body in charge of the long-term management of all radioactive waste, under the supervision of the Ministry of Ecology, Energy, Sustainable Development and the Sea (formerly the Ministry of Industry and the Ministry of Environment), and the Ministry of Research. The Andra operates two storage centers in the Aube region (France): the center for short-lived low- and intermediate-level wastes, and the center for very-low-level radioactive wastes. This document is the 2009 activity report of the center for short-lived low- and intermediate-level wastes. It presents a review of the activities of the center: presentation of the installations, safety and radiation protection, events or incidents, environmental monitoring, wastes management, public information, opinion of the Health and safety Committee (CHSCT)

  3. Aube storage center for short-lived low- and intermediate-level wastes. Annual report 2008

    International Nuclear Information System (INIS)

    2009-06-01

    The National Radioactive Waste Management Agency (Andra), was established by the December 1991 Waste Act as a public body in charge of the long-term management of all radioactive waste, under the supervision of the Ministry of Ecology, Energy, Sustainable Development and the Sea (formerly the Ministry of Industry and the Ministry of Environment), and the Ministry of Research. The Andra operates two storage centers in the Aube region (France): the center for short-lived low- and intermediate-level wastes, and the center for very-low-level radioactive wastes. This document is the 2008 activity report of the center for short-lived low- and intermediate-level wastes. It presents a review of the activities of the center: presentation of the installations, safety and radiation protection, events or incidents, environmental monitoring, wastes management, public information

  4. Aube storage center for short-lived low- and intermediate-level wastes. Annual report 2010

    International Nuclear Information System (INIS)

    2011-06-01

    The National Radioactive Waste Management Agency (Andra), was established by the December 1991 Waste Act as a public body in charge of the long-term management of all radioactive waste, under the supervision of the Ministry of Ecology, Energy, Sustainable Development and the Sea (formerly the Ministry of Industry and the Ministry of Environment), and the Ministry of Research. The Andra operates two storage centers in the Aube region (France): the center for short-lived low- and intermediate-level wastes, and the center for very-low-level radioactive wastes. This document is the 2010 activity report of the center for short-lived low- and intermediate-level wastes. It presents a review of the activities of the center: presentation of the installations, safety and radiation protection, events or incidents, environmental monitoring, wastes management, public information, recommendations of the Health and safety Committee (CHSCT)

  5. Simulation Studies of Diffusion-Release and Effusive-Flow of Short-Lived Radioactive Isotopes

    CERN Document Server

    Zhang, Yan; Kawai, Yoko

    2005-01-01

    Delay times associated with diffusion release from targets and effusive-flow transport of radioactive isotopes to ion sources are principal intensity limiters at ISOL-based radioactive ion beam facilities, and simulation studies with computer models are cost effective methods for designing targets and vapor transport systems with minimum delay times to avoid excessive decay losses of short lived ion species. A finite difference code, Diffuse II, was recently developed at the Oak Ridge National Laboratory to study diffusion-release of short-lived species from three principal target geometries. Simulation results are in close agreement with analytical solutions to Fick’s second equation. Complementary to the development of Diffuse II, the Monte-Carlo code, Effusion, was developed to address issues related to the design of fast vapor transport systems. Results, derived by using Effusion, are also found to closely agree with experimental measurements. In this presentation, the codes will be used in conc...

  6. Nuclear fall-out shelter

    International Nuclear Information System (INIS)

    Lowery, R.J.

    1981-01-01

    An underground nuclear fall-out shelter has a plastics shell which, apart from service and access openings, is waterproof and provided, if desired, with a concrete roof. The shelter has an access opening, an air system, lighting, water storage, sanitation and sewage facilities. (author)

  7. Dynamical Detection of Topological Phase Transitions in Short-Lived Atomic Systems

    OpenAIRE

    Setiawan, F.; Sengupta, K.; Spielman, I. B.; Sau, Jay D.

    2015-01-01

    We demonstrate that dynamical probes provide direct means of detecting the topological phase transition (TPT) between conventional and topological phases, which would otherwise be difficult to access because of loss or heating processes. We propose to avoid such heating by rapidly quenching in and out of the short-lived topological phase across the transition that supports gapless excitations. Following the quench, the distribution of excitations in the final conventional phase carries signat...

  8. Extrinsic and intrinsic factors that shape the life history of the short living scallop Argopecten ventricosus

    OpenAIRE

    Guerra, Citlali

    2011-01-01

    The scallop Argopecten ventricosus is characterized by its high swimming activity, fast growth, high reproductive effort and the early age to get first sexual maturity. These traits may be the result of the adaptation to a specific environment that favors an active lifestyle and a short lifespan (2 years). This opens the question of how environmental factors modulate the way a short living marine ectotherm budget energy investments among life history traits and how this modulation impacts the...

  9. Place of the final disposal of short lived dismantling waste; Plats foer slutfoervaring av kortlivat rivningsavfall

    Energy Technology Data Exchange (ETDEWEB)

    NONE

    2013-01-15

    This report deals with the short-lived low and intermediate level radioactive waste, which will mainly arise from the dismantling of the Swedish nuclear power plants, but also the dismantling of other nuclear facilities. For these installations to be dismantled, there must be the capacity to receive and dispose of dismantling waste. SKB plans to expand the existing final repository for short-lived radioactive waste (SFR) in Forsmark for this purpose. The legislation requires alternatives to the chosen location. The alternate location for the disposal of decommissioning waste SKB has chosen to compare with is a location in the Simpevarp area outside Oskarshamn. There are currently Oskarshamn nuclear power plant and SKB between stock 'CLAB'. The choice of Simpevarp as alternative location is based on that it's one of the places in the country where data on the bedrock is available to an extent that allows an assessment of the prospects for long-term security, such an assessment is actually showing good potential, and that the location provide realistic opportunities to put into practice the disposal of decommissioning waste. At a comparison between the disposal of short-lived decommissioning waste in an extension of SFR with the option to build a separate repository for short-lived decommissioning waste in Simpevarp, the conclusion is that both options offer potentially good prospects for long-term security. The differences still indicated speaks to the Forsmark advantage. Similar conclusions were obtained when comparing the factors of environment, health and social aspects.

  10. Identification of short-lived neutron-rich ruthenium and rhodium isotopes in fission

    International Nuclear Information System (INIS)

    Franz, G.; Herrmann, G.

    1975-01-01

    Short-lived ruthenium and rhodium isotopes ( 107 Ru, 108 Ru, 108 Rh, 109 Ru, 109 Rh, 110 Ru, 110 Rh, 111 Ru, 111 Rh, 112 Ru, 112 Rh, 113 Ru) have been separated from fission products by a rapid chemical procedure and identified by means of γ-ray spectroscopy. Nuclides with half-lives down to 3 sec were accessible. Ruthenium isotopes up to mass number 113 have been identified. (author)

  11. Last developments in the Belgian disposal programme for low and intermediate short-lived waste

    International Nuclear Information System (INIS)

    Boyazis, Jean-Paul

    2006-01-01

    After an historical reminder of the several phases of the Belgian program for the disposal of low and medium level short-lived waste since the creation of ONDRAF/NIRAS and the bad results obtained in the 90's by using a pure technical approach, the presentation will explain the main lines of the new methodology developed, as a consequence of the government decision of 16 January 1998 in ONDRAF/NIRAS to improve local acceptance for the disposal project. The way local partnerships were created with four nuclear municipalities under the form of a non-profit organization with a clear mission, the functioning, on a voluntary base, of the different partnerships during four to six years and the concrete results obtained until now using this very innovative method will be addressed. The last developments of the Belgian program for the disposal of low and medium level and short-lived waste will be presented, including the recent and very important decision of the Belgian government of 23 June 2006 to dispose of the low and medium active short-lived waste in a surface disposal installation on the territory of the municipality Dessel. (author)

  12. Applications of short lived nuclides in activation analysis, problems and progress

    Energy Technology Data Exchange (ETDEWEB)

    Grass, F [Atominstitut, Vienna (Austria)

    1976-07-01

    Short lived nuclides or isomeric transitions, respectively would have some advantages over long lived ones. Although we published a paper concerning a germanium-determination in iron meteorites some years ago, only few laboratories use this technique, the main reason being that the high matrix activity disturbs the measurement of energy-spectra. A multichannel analyzer in the time sequence mode enables Li-8 determination by a purely instrumental method which is therefore used more frequently. In the time sequence mode much higher counting rates up to 10 - 50 MHz are processed then by taking energy-spectra. This is the reason why activation analysis with short lived isomeric states is seldom applied when counting rate and pulse height are to be detected simultaneously. Exceptional difficulties are encountered in measurement of samples activated by a reactor pulse. Further difficulties arise from the fact that an optimal expelling time depends on the half life of the nuclide, and is more critical if the half life is short and the full width half maximum of the reactor pulse is small. Commercial Ge-Li-detectors can be used only at low counting rates, so that samples with high matrix activities cannot be measured. Modifying the electronic system enables registration of samples with high matrix activities. For short lived nuclides emitting hard beta-rays, e.g. B-12 or Li-8, a Cerenkov-detector is optimal. These problems are discussed in examples. (author)

  13. Design and development of a computer-based continuous monitor for the determination of the short-lived decay products of radon and thoron

    Energy Technology Data Exchange (ETDEWEB)

    Bigu, J [Department of Energy, Mines and Resources, Elliot Lake, Ontario (Canada). Elliot Lake Lab.; Raz, R; Golden, K; Dominguez, P [Alpha-NUCLEAR, Toronto, Ontario (Canada)

    1984-08-15

    A portable, rugged, monitor has been designed and built for measuring the short-lived decay products of radon and thoron. The monitor is computer-based and employs a continuous filter strip which can be advanced at programmable time intervals to allow unattended continuous operation with automatic sampling, analysis and recording of radiation levels. Radionuclide analysis is carried out by two silicon diffused-junction alpha-detectors and electronic circuitry with multichannel spectral analysis capabilities. Standard gross ..cap alpha..-count methods and ..cap alpha..-spectroscopy methods can easily be implemented. The built-in computer performs a variety of operations via a specially designed interface module, including control and data recording functions, and computations, program storage and display functions. Programs and data are stored in the built-in casette tape drive and the computer integrated CRT display and keyboard allow simple, prompted menu-type operation of standard software. Graphical presentation of ..cap alpha..-spectra can be shown on the computer CRT and printed when required on the computer built-in thermal printer. In addition, to implementing the specially developed radionuclide analysis software, the operator can interact and modify existing software, and program new ones, through BASIC language programming, or employ the computer in a totally unrelated, general purpose model. Although the monitor is ideally suited for environmental radon (thoron) daughter monitoring, it could also be used in the determination of other airborne radionuclides provided adequate analytical procedures are developed or included in the already existing computer software.

  14. Design and development of a computer-based continuous monitor for the determination of the short-lived decay products of radon and thoron

    International Nuclear Information System (INIS)

    Bigu, J.

    1984-01-01

    A portable, rugged, monitor has been designed and built for measuring the short-lived decay products of radon and thoron. The monitor is computer-based and employs a continuous filter strip which can be advanced at programmable time intervals to allow unattended continuous operatin with automatic sampling, analysis and recording of radiation levels. Radionuclide analysis is carried out by two silicon diffused-junction alpha-detectors and electronic circuitry with multichannel spectral analysis capabilities. Standard gross α-count methods and α-spectroscopy methods can easily be implemented. The built-in computer performs a variety of operations via a specially designed interface module, including control and data recording functions, and computations, program storage and display functions. Programs and data are stored in the built-in casette tape drive and the computer integrated CRT display and keyboard allow simple, prompted menu-type operation of standard software. Graphical presentation of α-spectra can be shown on the computer CRT and printed when required on the computer built-in thermal printer. In addition, to implementing the specially developed radionuclide analysis software, the operator can interact and modify existing software, and program new ones, through BASIC language programming, or employ the computer in a totally unrelated, general purpose model. Although the monitor is ideally suited for environmental radon (thoron) daughter monitoring, it could also be used in the determination of other airborne radionuclides provided adequate analytical procedures are developed or included in the already existing computer software. (orig.)

  15. The uptake of radionuclides by plants

    International Nuclear Information System (INIS)

    Cawse, P.A.; Turner, G.S.

    1982-02-01

    A review of the literature, since 1970, on the research into the uptake of radionuclides by plants, with references to earlier soil and plant studies on the fate of nuclear weapons fallout. Experimental data on the uptake of plutonium isotopes, americium 241, cesium 137, radium 226, curium 244 and neptunium 237 and details of the chemical form of the radionuclide, soil type and plant growth period are tabulated. (U.K.)

  16. Radiation Doses to Members of the U.S. Population from Ubiquitous Radionuclides in the Body: Part 3, Results, Variability, and Uncertainty

    International Nuclear Information System (INIS)

    Watson, David J.; Strom, Daniel J.

    2011-01-01

    This paper is part three of a three-part series investigating annual effective doses to residents of the United States from intakes of ubiquitous radionuclides, including radionuclides occurring naturally, radionuclides whose concentrations are technologically enhanced, and anthropogenic radionuclides. The radionuclides of interest are the 238 U series (14 nuclides), the actinium series (headed by 235 U; 11 nuclides), and the 232 Th series (11 nuclides); primordial radionuclides 87 Rb and 40 K; cosmogenic and fallout radionuclides 14 C and 3 H; and purely anthropogenic radionuclides 137 Cs- 137m Ba, 129 I and 90 Sr- 90 Y. This series of papers explicitly excludes intakes from inhaling 222 Rn, 220 Rn, and their short-lived decay products; it also excludes intakes of radionuclides in occupational and medical settings. Part one reviewed, summarized, characterized, and grouped all published and some unpublished data for U.S. residents on ubiquitous radionuclide concentrations in tissues and organs. Part two described the methods used to organize the data collected in part one and segregate it into the ages and genders defined by the study, imputed missing values from the existing data, apportioned activity in bone, and imputed activity in hollow organ contents and the remainder of the body. This paper estimates equivalent doses to target tissues from source regions and maps target tissues to lists of tissues with International Commission on Radiation Protection (ICRP) tissue-weighting factors or to surrogate tissue regions when there is no direct match. Effective doses, using ICRP tissue-weighting factors recommended in 1977, 1990, and 2007, are then calculated, and an upper bound of variability of the effective dose is estimated by calculating the average coefficients of variation (CV), assuming all variance is due to variability. Most of the data were for adult males, whose average annual effective dose is estimated to be 337 (micro)Sv y -1 (CV = 0.65, geometric mean

  17. Improving weapons fallout time series on a global basis using precipitation data

    International Nuclear Information System (INIS)

    Palsson, S.E.; Howard, B.J.; Aoyama, M.

    2004-01-01

    The fallout from the atmospheric weapons tests in the late fifties and early sixties forms the main source of man made radionuclides in the terrestrial environment. It is important to be able to distinguish global fallout from other sources of man-made radioactivity, and therefore to have good methods of quantifying the level of global fallout in areas where it has not previously been measured. Because global fallout was deposited over many years, model validation can require knowledge about deposition time series which are not available through direct measurements. This can be especially important for sparsely populated areas with vulnerable ecosystems, where high transfer of radionuclides, particularly radiocaesium, may occur. The UNSCEAR reports describe the global data and show how the deposition was dependent on latitude. Others have successfully used a model assuming a proportional relationship between deposition and precipitation (e.g. on a regional scale within the AMAP project and on a local scale in some countries, such as Iceland and Sweden). This paper describes a study where different data sets were combined to test, at a local scale to a global scale, how well the proportional relationship between precipitation and deposition holds and to what degree other effects (e.g. dependence on latitude as in the UNSCEAR model) need to be taken into account. It makes use of the Integrated Global Fallout Database of the Meteorological Research Institute of Japan which has been used previously to demonstrate the relationship between precipitation and deposition and subsequently to make an estimate of the total fallout amount of 137 Cs in the mid latitudes of the Northern Hemisphere. The study described in this paper provides a fuller description of global deposition than the latitude or precipitation based studies alone. Applied in a simple model as presented here, this enable better deposition estimation (including time dependency), especially if precipitation

  18. The choice between Ruark-Devol and Poisson statistics in the measurement of short-lived radionuclides

    International Nuclear Information System (INIS)

    Kennedy, G.

    1981-01-01

    The question of whether to use Poisson or Ruark-Devol statistics for radioactivity measurements in which the counting time is long compared to the half-life is discussed. Experimental data are presented which are well described by Poisson statistics. The applications of Ruark-Devol statistics are found to be very limited, in disagreement with earlier publications. (author)

  19. Laser spectroscopy of short-lived radionuclides in an ion trap: MIRACLS’ proof-of-principle experiment

    CERN Document Server

    Maier, Franziska Maria

    2017-01-01

    Since 1978 Collinear Laser Spectroscopy is done at COLLAPS [1], which is located at ISOLDE,CERN’sfacilityforsynthesizingradioactiveions,toexplorethenuclearshell structure of the most exotic atomic nuclides far away from stability. At COLLAPS a laser beam is overlapped with a radioactive ion beam. If the wavelength of the laser corresponds to the energy difference of the electronic transitions, the laser excites the ions. The excited ions decay back to the ionic ground state and emit fluorescence photons that can be detected with photomultiplier tubes (PMTs). By measuring the hyperfine structure of the involved ionic states one obtains information about the nuclear spin, the nuclear magnetic dipole moment and the nuclear electric quadrupole moment. This hyperfine splitting is caused by the interaction of the bound electrons withtheatomicnucleus. Theelectronsinduceanelectromagneticfieldattheplaceof the nucleus that interacts with the electromagnetic nuclear moments and the nuclear spin. By calculating th...

  20. Short lived radionuclides in gases and magmas: contribution to the study of degassing and of the dynamics of magmatic reservoirs

    International Nuclear Information System (INIS)

    Gauthier, P.J.

    1998-01-01

    Crystallization and magma degassing at Stromboli (Italy) and Merapi (Indonesia) volcanoes are studied through 230 Th- 226 Ra- 210 Pb and 210 Pb- 210 Bi- 210 Po disequilibria in lavas and gases. An attempt to date crystallization by internal isochrones in ( 226 Ra)/Ba - ( 230 Th)/Ba and ( 210 Pb)/Pb - ( 226 Ra)/Pb diagrams reveals the complex evolution of these arc magmas. Several models (instantaneous but non simultaneous crystallization of the different mineral phases; continuous crystallization) are proposed to explain the lack of simple isochrones. The influence of other magmatic processes (assimilation, magma reinjection, degassing...) is discussed. The role played by radon loss from magmas (controlled by the ex solution of major gas species) on 210 Pb- 226 Ra disequilibria in lavas is examined through a model of dynamic degassing. At Stromboli, the magma reservoir has reached a steady-state and is rapidly renewed, thus explaining (Pb/Ra) ratios close to 1. At Merapi, the evolution of the reservoir is controlled by a succession of low dynamics degassing periods ( 2 analyses in the volcanic plume. The contribution of Etna as a source of atmospheric pollution is estimated during periods of contrasted volcanic activity and is compared to the volcanic emissions worldwide. (author)

  1. How do radionuclides behave in soils

    Energy Technology Data Exchange (ETDEWEB)

    Gerzabek, M

    1986-01-01

    The surface fallout of J, Cs, Ru, Sr and Pu after Chernobyl is given in a table. Another table indicates activities of J, Cs and Ru measured in the soil at different depths up to 200mm. Comments are given on the mobility and spread of radionuclides in the soil. (G.Q.).

  2. Cesium, iodine and tritium in NW Pacific waters - a comparison of the Fukushima impact with global fallout

    DEFF Research Database (Denmark)

    Povinec, P. P.; Aoyama, M.; Biddulph, D.

    2013-01-01

    Radionuclide impact of the Fukushima Dai-ichi nuclear power plant accident on the distribution of radionuclides in seawater of the NW Pacific Ocean is compared with global fallout from atmospheric tests of nuclear weapons. Surface and water column samples collected during the Ka’imikai-o-Kanaloa ......Radionuclide impact of the Fukushima Dai-ichi nuclear power plant accident on the distribution of radionuclides in seawater of the NW Pacific Ocean is compared with global fallout from atmospheric tests of nuclear weapons. Surface and water column samples collected during the Ka......-derived radionuclides downward to the depth of 300m has already occurred. The observed 137Cs levels in surface waters and in the water column are compared with predictions obtained from the ocean general circulation model, which indicates that the Kuroshio Current acts as a southern boundary for the transport...... the coast, where all three radionuclides were analyzed, the Fukushima impact on the levels of these three radionuclides represents an increase above the global fallout background by factors of about 1000, 50 and 3, respectively. The water column data indicate that the transport of Fukushima...

  3. Systematic measurement of beta-decay half-lives of short-lived isotopes

    Energy Technology Data Exchange (ETDEWEB)

    Hirose, T.; Yamamoto, H.; Kawade, K. [Nagoya Univ. (Japan); Iida, T.; Takahashi, A.; Kasugai, Y.; Ikeda, Y.

    1997-03-01

    We have measured the half-lives of short-lived isotopes for past decade and deduced the half-lives of 6 isotopes further. These results demonstrated that most of the literature values shorter than 10 min systematically deviated from our measurement ones. The cause seems to be that a large number of the previous half-life studies were performed with scintillation counters before 1970 and they had a difficulty in distinguishing the interest {gamma}-ray from the contamination and correcting for pile-up and dead-time losses. Moreover, the deviated data found to be quoted for evaluation. (author)

  4. Quantum non-locality in a two-slit interferometer for short-lived particles

    International Nuclear Information System (INIS)

    Klein, Spencer R.; Nystrand, Joakim

    2001-01-01

    We describe a new test of quantum nonlocality, using an interferometer for short-lived particles. The separation is large compared with the particle lifetimes. This interferometer is realized by vector meson production in distant heavy ion collisions. The mesons decay before waves from the two sources (ions) can overlap, so interference is only possible among the decay products. The post-decay wave function must retain amplitudes for all possible decays. The decay products are spatially separated, necessitating a non-local wave function. The interference is measurable by summing the product momenta. Alternately, the products positions could be observed, allowing new tests of the EPR paradox

  5. Short-lived cyclotron-produced radioisotopes: Medi-Physics, Inc.'s commitment

    International Nuclear Information System (INIS)

    Kramer, H.H.

    1985-01-01

    Medi-Physics, Inc., is a major US supplier of short-lived cyclotron-produced radioisotopes for radiopharmaceuticals, as well as routinely producing and distributing the greatest number of 123 I radiopharmaceuticals. The present commercial production capacity for 123 I is more than ten times the theoretical need for existing procedures and is more than adequate for the research and development of new radiopharmaceuticals. However, production capacity is only one component of many that are required to supply a radioisotope for human use. These components are summarized in this paper

  6. Rapid transfer of short-lived radioisotopes via a 2. 4 km rabbit system

    Energy Technology Data Exchange (ETDEWEB)

    Burgerjon, J J; Gelbart, Z; Lau, V; Lehnart, D; Lenz, J; Pate, B D; Ruth, T J; Sprenger, H P; van Oers, N S.C.

    1984-09-01

    A 2.4 km long pipeline between a cyclotron and a hospital is used for the rapid transfer of short-lived radiopharmaceuticals. The vials containing the pharmaceuticals are placed inside capsules (rabbits) that are blown through a tube by means of compressed air. Travel times as short as 2 min are achieved, which makes the system suitable for the transfer of /sup 15/O, which has a 2 min half-life. The construction and test results of the system are described along with a computer model, developed to explain some properties of the system. 7 references, 15 figures, 2 tables.

  7. [Hyperfine structure and isotope shift measurements of short lived elements by laser spectroscopy

    International Nuclear Information System (INIS)

    Schuessler, H.A.

    1986-01-01

    The aim of this research is to determine nuclear moments and charge distributions of short-lived isotopes produced both on-line and off-line to a nuclear facility. These measurements give detailed information on the nuclear force and are used to test current nuclear models. The small amounts of nuclei which can be produced off stability constitute the challenge in these experiments. Presently mainly neutron-rich isotopes are being studied by three ultrasensitive high-resolution laser techniques. These are collinear fast ion-beam laser spectroscopy, stored-ion laser spectroscopy and fluorescence spectroscopy. 5 figs

  8. Preparing isomerically pure beams of short-lived nuclei at JYFLTRAP

    Energy Technology Data Exchange (ETDEWEB)

    Eronen, T. [Department of Physics, University of Jyvaeskylae, P.O. Box 35 (YFL), FIN-40014 (Finland)], E-mail: tommi.eronen@jyu.fi; Elomaa, V.-V.; Hager, U.; Hakala, J.; Jokinen, A.; Kankainen, A.; Rahaman, S.; Rissanen, J.; Weber, C.; Aystoe, J. [Department of Physics, University of Jyvaeskylae, P.O. Box 35 (YFL), FIN-40014 (Finland)

    2008-10-15

    A new procedure to prepare isomerically clean samples of short-lived ions with a mass resolving power of more than 1 x 10{sup 5} has been developed at the JYFLTRAP tandem Penning trap system. The method utilises a dipolar rf-excitation of the ion motion with separated oscillatory fields in the precision trap. During a subsequent retransfer to the purification trap, the contaminants are rejected and as a consequence, the remaining bunch is isomerically cleaned. This newly-developed method is suitable for very high-resolution cleaning and is at least a factor of five faster than the methods used so far in Penning trap mass spectrometry.

  9. PATHWAY: a simulation model of radionuclide-transport through agricultural food chains

    International Nuclear Information System (INIS)

    Kirchner, T.B.; Whicker, F.W.; Otis, M.D.

    1982-01-01

    PATHWAY simulates the transport of radionuclides from fallout through an agricultural ecosystem. The agro-ecosystem is subdivided into several land management units, each of which is used either for grazing animals, for growing hay, or for growing food crops. The model simulates the transport of radionuclides by both discrete events and continuous, time-dependent processes. The discrete events include tillage of soil, harvest and storage of crops,and deposition of fallout. The continuous processes include the transport of radionuclides due to resuspension, weathering, rain splash, percolation, leaching, adsorption and desorption of radionuclides in the soil, root uptake, foliar absorption, growth and senescence of vegetation, and the ingestion assimilation, and excretion of radionuclides by animals. Preliminary validation studies indicate that the model dynamics and simulated values of radionuclide concentrations in several agricultural products agree well with measured values when the model is driven with site specific data on deposition from world-wide fallout

  10. Production of Short-Lived Radionuclides at the Hahn-Meitner Institute in West Berlin; Production de Radionuclides a Courte Periode a l'Institut Hahn-Meitner de Berlin-Ouest; ПРОИЗВОДСТВО КОРОТКОЖИВУЩИХ РАДИОИЗОТОПОВ В ИНСТИТУТЕ ХАНА-МАЙТНЕРА В ЗАПАДНОМ БЕРЛИНЕ; Produccion de Radionuclidos de Periodo Corto en el Instituto Hahn-Meitner de Berlin Occidental

    Energy Technology Data Exchange (ETDEWEB)

    Felix, F. W.; Pirrwitz, D.; Szabo de Bucs, E. [Hahn - Meitner-Institut fuer Kern Forschung, Berlin, Federal Republic of Germany (Germany)

    1963-03-15

    The Hahn-Meitner Institute for Nuclear Research has produced short-lived radionuclides for medical and scientific purposes in the West Berlin area since 1960. Production now covers, the nuclides commonly used in medical applications, such as Na{sup 25}, K{sup 42} and Au{sup 198}, and other outstanding nuclides such as Cu{sup 64}, Zn{sup 69m} and F{sup 18}; Na{sup 24} and K{sup 42}are produced by neutron irradiation of the chlorides and, after calibration, distributed as solid material; Au{sup 198} is irradiated in metallic form, which is suitable for implantation in cancer therapy; F{sup 18} is produced by the reaction 0{sup 16} (t, n) and irradiation of LiNO{sub 3}. The separation of F{sup 18} by ion exchange showed better results than those usually given in the literature. For the production of Cu{sup 64} and Zn{sup 69m} special electrolytic methods have been developed to extract the radionuclides produced by a Szilard- Chalmers reaction on the phthalocyanines. Both nuclides have found application in medical diagnostics. In the paper details are given of irradiation facilities and techniques, production methods and apparatus, essay and calibration of the radionuclides produced and production capacity. (author) [French] Depuis 1960, l'Institut de recherches nucleaires Hahn-Meitner produit des radionucleides a courte periode a usage medical et scientifique pour la region de Berlin-Ouest. L'Institut prepare maintenant des nucleides utilises couramment en medecine tels que {sup 25}Na, {sup 42}K et {sup 198}Au, ainsi que quelques autres nucleides moins usuels comme {sup 64}Cu, {sup 69m}Zn et {sup 18}F. Le sodium-24 et le potassium-42 sont produits par irradiation neu- tronique des chlorures et distribues sous forme solide apres etalonnage. L'or-198 est irradie sous forme metallique, utilisable pour les implantations dans le traitement du cancer. Le fluor-18 est produit par la reaction {sup 16}0 (t, n) et par irradiation de LiNO{sub 3}. La separation de {sup 18}F par

  11. Nuclear Fallout Decision Tool for First Responders

    Energy Technology Data Exchange (ETDEWEB)

    Archibald, E. J. [Lawrence Livermore National Lab. (LLNL), Livermore, CA (United States); Buddemeier, B. R. [Lawrence Livermore National Lab. (LLNL), Livermore, CA (United States)

    2010-08-11

    If terrorists detonated an improvised nuclear device (IND) in an urban area, thousands of people would die from the blast, and many more would become sick or die from exposure to fallout radiation. Proper sheltering and evacuation can protect people from fallout and save lives. This project provides guidance to first responders as to when to evacuate and what route to take to protect themselves against fallout radiation.

  12. Short-lived radioactive nuclides in meteorites and early solar system processes

    International Nuclear Information System (INIS)

    Chaussidon, M.; Gounelle, M.

    2007-01-01

    Now extinct, short-lived radioactive nuclides, such as 7 Be (T 1/2 = 53 days), 10 Be (T 1/2 = 1.5 Ma), 26 Al (T 1/2 = 0.74 Ma), 36 Cl (T 1/2 = 0.3 Ma), 41 Ca (T 1/2 = 0.1 Ma), 53 Mn (T 1/2 = 3.7 Ma) and 60 Fe (T 1/2 = 1.5 Ma), were present in the proto-solar nebula when the various components of meteorites formed. The presence of these radioactive isotopes requires a 'last-minute' origin, either nucleosynthesis in a massive star dying close in space and time to the nascent solar system or production by local irradiation of part of the proto-solar disk by high-energy solar cosmic rays. In this review, we list: (i) the different observations indicating the existence of multiple origins for short-lived radioactive nuclides, namely 7 Be, 10 Be and 36 Cl for irradiation scenario and 60 Fe for injection scenario; (ii) the constraints that exist on their distribution (homogeneous or heterogeneous) in the accretion disk; (iii) the constraints they brought on the timescales of nebular processes (from Ca-Al-rich inclusions to chondrules) and of the accretion and differentiation of planetesimals. (authors)

  13. Behaviour of short-lived fission products within operating UO2 fuel elements

    International Nuclear Information System (INIS)

    Hastings, I.J.; Hunt, C.E.L.; Lipsett, J.J.

    1983-01-01

    We have carried out experiments using a ''sweep gas'' technique to determine the behaviour of short-lived fission products within operating, intact UO 2 fuel elements. The Zircaloy-4-clad elements were 500 mm long and contained fuel of density 10.65-10.71 Mg/m 3 . A He-2% H 2 carrier gas swept gaseous or volatile fission products out of the operating fuel element past a gamma spectrometer for measurement. In tests at linear powers of 45 and 60 kW/m to maximum burnups of 70 MW.h/kg U, the species measured directly at the spectrometer were generally the short-lived xenons and kryptons. We did not observe iodine or bromine during normal operation. However, we have deduced the behaviour of I-133 and I-135 from the decay of Xe-133 and Xe-135 during reactor shutdowns. Plots of R/B (released/born) against lambda (decay constant) or effective lambda for all isotopes observed at 45 and 60 kW/m show that a line of slope -0.5, corresponding with diffusion kinetics, is a good fit to the measured xenon and krypton data. Our inferred release of iodine fits the same line. From this we can extrapolate to an R/B for I-131 of about 5x10 -3 . The ANS 5.4 release correlation gives calculated results in good agreement with our measurements. (author)

  14. Search for short-lived particles produced on nuclei with a heavy liquid mini bubble chamber

    CERN Multimedia

    2002-01-01

    The aim of this experiment is to search for short-lived particles produced in hadronic interactions on nuclei with our high resolution heavy liquid mini bubble chamber BIBC, aiming to establish the cross-section for associated production in hadron-nucleus collisions, its $A$-dependence and an approximate value of the lifetime. The chamber will be operated at a bubble density of 290 bubbles/cm and with an apparent bubble size of 30 $\\mu$m in real space. In test runs at CERN we measured detection efficiencies which, together with simulations of $D\\bar{D}$ production and decay, lead to a sensitivity of 0.25 events/($\\mu$b/N) per day if the lifetime is of the order of $5\\times10^{-13}$s. A null result after 10 days running time would set an upper limit on the production cross section to $3 \\mu$b. \\\\ \\\\ In order to measure the momenta of charged decay products of short-lived particles, the bubble chamber will be placed 1.80 m upstream of the streamer chamber of the NA5 experiment (MPI). The geometrical acceptance ...

  15. Continuous administration of short-lived radioisotope tracers and the analogous Laplace transform

    International Nuclear Information System (INIS)

    Orr, J.S.

    1979-01-01

    Short-lived radioactive tracers are used because of the low radiation dose to patients. Another advantage finding increasing use, however, is that the equilibrium activities achieved by continuous administration to a steady state contain kinetic information. This is not the case with long-lived isotopes. The derivation of quantitative kinetic information in the form of rate constants or flows requires the formulation of a model of the system being studied. Several approaches to this have been published based on a model of single compartments with simultaneous arrival of tracer. To deal with more realistic models a method is proposed which uses the analogy between the procedure of continuous administration of short-lived tracer and the Laplace transform. This analogy permits all the theorems of Laplace transform theory to be applied to the analysis of measured activities. The basis of the analogy is explained and examples are given of its application to a number of models which represent actual physiology more realistically than single compartment models. In these applications the transformed equations representing the model, with measured values of activity inserted for each transform, are solved to derive the rate constants. This is different from the use of Laplace transforms where the constant coefficients are known and the initial value problem is solved to find the behaviour of the variables. (author)

  16. Production of exotic, short lived carbon isotopes in ISOL-type facilities

    CERN Document Server

    Franberg, Hanna; Köster, Ulli; Ammann, Markus

    2008-01-01

    The beam intensities of short-lived carbon isotopes at Isotope Separation On-Line (ISOL) facilities have been limited in the past for technical reasons. The production of radioactive ion beams of carbon isotopes is currently of high interest for fundamental nuclear physics research. To produce radioactive ions a target station consisting of a target in a container connected to an ion source via a transfer line is commonly used. The target is heated to vaporize the product for transport. Carbon in elementary form is a very reactive element and react strongly with hot metal surfaces. Due to the strong chemisorption interaction, in the target and ion source unit, the atoms undergo significant retention on their way from the target to the ion source. Due to this the short lived isotopes decays and are lost leading to low ion yields. A first approach to tackle these limitations consists of incorporating the carbon atoms into less reactive molecules and to use materials for the target housing and the transfer line ...

  17. Short-lived pollutants in the Arctic: their climate impact and possible mitigation strategies

    Directory of Open Access Journals (Sweden)

    S. Menon

    2008-03-01

    Full Text Available Several short-lived pollutants known to impact Arctic climate may be contributing to the accelerated rates of warming observed in this region relative to the global annually averaged temperature increase. Here, we present a summary of the short-lived pollutants that impact Arctic climate including methane, tropospheric ozone, and tropospheric aerosols. For each pollutant, we provide a description of the major sources and the mechanism of forcing. We also provide the first seasonally averaged forcing and corresponding temperature response estimates focused specifically on the Arctic. The calculations indicate that the forcings due to black carbon, methane, and tropospheric ozone lead to a positive surface temperature response indicating the need to reduce emissions of these species within and outside the Arctic. Additional aerosol species may also lead to surface warming if the aerosol is coincident with thin, low lying clouds. We suggest strategies for reducing the warming based on current knowledge and discuss directions for future research to address the large remaining uncertainties.

  18. Short-lived pollutants in the Arctic: their climate impact and possible mitigation strategies

    Energy Technology Data Exchange (ETDEWEB)

    Menon, Surabi; Quinn, P.K.; Bates, T.S.; Baum, E.; Doubleday, N.; Fiore, A.M.; Flanner, M.; Fridlind, A.; Garrett, T.J.; Koch, D.; Menon, S.; Shindell, D.; Stohl, A.; Warren, S.G.

    2007-09-24

    Several short-lived pollutants known to impact Arctic climate may be contributing to the accelerated rates of warming observed in this region relative to the global annually averaged temperature increase. Here, we present a summary of the short-lived pollutants that impact Arctic climate including methane, tropospheric ozone, and tropospheric aerosols. For each pollutant, we provide a description of the major sources and the mechanism of forcing. We also provide the first seasonally averaged forcing and corresponding temperature response estimates focused specifically on the Arctic. The calculations indicate that the forcings due to black carbon, methane, and tropospheric ozone lead to a positive surface temperature response indicating the need to reduce emissions of these species within and outside the Arctic. Additional aerosol species may also lead to surface warming if the aerosol is coincident with thin, low lying clouds. We suggest strategies for reducing the warming based on current knowledge and discuss directions for future research to address the large remaining uncertainties.

  19. Radionuclide production and radiopharmaceutical chemistry with BNL cyclotrons

    International Nuclear Information System (INIS)

    Lambrecht, R.M.; Wolf, A.P.

    1985-01-01

    The Brookhaven National Laboratory (BNL) radiopharmaceutical chemistry program focuses on production and utilization of radionuclides having a half-life of > 2 hr. However, a major portion of the BNL program is devoted to short-lived radionuclides, such as 11 C and 18 F. Activities encompassed in the program are classified into seven areas: cyclotron parameters, radiochemistry, design and rapid synthesis of radiopharmaceuticals and labeled compounds, radiotracer evaluation in animals, studies in humans, technology transfer, and several other areas

  20. Erosional losses of fallout plutonium

    International Nuclear Information System (INIS)

    Foster, G.R.; Hakonson, T.E.

    1987-01-01

    Plutonium from fallout after atmospheric explosion of nuclear weapons in the 1950's and 1960s is being redistributed over the landscape by soil erosion and carried on sediment by streams to oceans. Erosion rates computed with the Universal Soil Loss Equation for more than 200,000 sample points on nonfederal land across the US were used to estimate plutonium removal rates by soil erosion. On the average, only about 4% of the eroded sediment reaches the outlet of a major river. The remaining sediment is deposited en route, and because deposition is a selective process, the sediment is enriched in fine particles having the highest concentration of plutonium because of the element's strong association with clay and silt-sized sediment. Estimated enrichment ratios, sediment delivery ratios, and erosion rates were used to estimate annual delivery of fallout plutonium. These estimates ranged from 0.002% of the initial fallout plutonium inventory for the Savannah River basin to 0.01% for the Columbia River basin, to 0.02% for the Hudson and Rio Grande River basins, to 0.08% for the Mississippi River basin. If the deposition of plutonium had been uniformly 1 mCi/km 2 , the estimated plutonium activity on suspended sediment would range from about 7 fCi/g of sediment of the Savannah River basin, to 9 fCi/g for the Mississippi River basin, to 12 fCi/g for the Hudson River basin, to 14 fCi/g for the Columbia and Rio Grande River basins. 45 references, 2 figures, 17 tables

  1. Fallout deposition in the Marshall Islands from Bikini and Enewetak nuclear weapons tests.

    Science.gov (United States)

    Beck, Harold L; Bouville, André; Moroz, Brian E; Simon, Steven L

    2010-08-01

    Deposition densities (Bq m(-2)) of all important dose-contributing radionuclides occurring in nuclear weapons testing fallout from tests conducted at Bikini and Enewetak Atolls (1946-1958) have been estimated on a test-specific basis for 32 atolls and separate reef islands of the Marshall Islands. A complete review of various historical and contemporary data, as well as meteorological analysis, was used to make judgments regarding which tests deposited fallout in the Marshall Islands and to estimate fallout deposition density. Our analysis suggested that only 20 of the 66 nuclear tests conducted in or near the Marshall Islands resulted in substantial fallout deposition on any of the 23 inhabited atolls. This analysis was confirmed by the fact that the sum of our estimates of 137Cs deposition from these 20 tests at each atoll is in good agreement with the total 137Cs deposited as estimated from contemporary soil sample analyses. The monitoring data and meteorological analyses were used to quantitatively estimate the deposition density of 63 activation and fission products for each nuclear test, plus the cumulative deposition of 239+240Pu at each atoll. Estimates of the degree of fractionation of fallout from each test at each atoll, as well as of the fallout transit times from the test sites to the atolls were used in this analysis. The estimates of radionuclide deposition density, fractionation, and transit times reported here are the most complete available anywhere and are suitable for estimations of both external and internal dose to representative persons as described in companion papers.

  2. Fallout forecasting: 1945-1962

    International Nuclear Information System (INIS)

    Kennedy, W.R. Jr.

    1986-03-01

    The delayed hazards of fallout from the detonations of nuclear devices in the atmosphere have always been the concern of those involved in the Test Program. Even before the Trinity Shot (TR-2) of July 16, 1945, many very competent, intelligent scientists and others from all fields of expertise tried their hand at the prediction problems. This resume and collection of parts from reports, memoranda, references, etc., endeavor to chronologically outline prediction methods used operationally in the field during Test Operations of nuclear devices fired into the atmosphere

  3. Radionuclides in the marine environment near the Farallon Islands

    International Nuclear Information System (INIS)

    Noshkin, V.E.; Wong, K.M.; Jokela, T.A.; Eagle, R.J.; Brunk, J.L.

    1978-01-01

    Isolated sediment areas containing plutonium and cesium radionuclide concentrations exceeding Pacific Ocean global radionuclide fallout levels have been reported in the Farallon Islands radioactive waste disposal area, west of San Francisco. We find the total 239+240 Pu and 137 Cs inventory of Farallon water columns to be within global fallout levels. The quantity of these radionuclides from nonfallout sources contaminating the sedimentary environment is unknown, but their contribution to the total water column inventory is insignificant compared with present fallout levels. Fish and invertebrates from the disposal region contain body burdens of 239+240 Pu and 137 Cs no greater than similar species exposed to global fallout. Within deep (2000 m) Farallon sediments, we do find that 238 Pu concentrations exceeding anticipated fallout levels are being remobilized to bottom waters. Fallout plutonium appears to be displaced laterally from the continental shelf down the slope into deeper offshore waters. Remobilized waste from the disposal site probably is displaced in the same manner

  4. Gold-195m short-lived single-photon emitter for cardiovascular studies

    International Nuclear Information System (INIS)

    Mena, I.; de Jong, R.; Mena, F.J.; Narahara, K.A.

    1985-01-01

    Ultrashort-lived radionuclides offer many advantages for clinical nuclear medicine. These radionuclide are generator-produced at bedside, with markedly diminished radiation exposure to the patient; larger doses of radionuclides can therefore be administered, and rapid, sequential, background-free studies can be performed. Gold-195m is an example of an ultrashort-lived radionuclide with a half-life of 30.4 sec. It is generated from /sup 195m/Hg (T/sub 1/2/, 40.6 hr). The quality of imaging and radiation exposure to patients is a function of the percentage breakthrough of /sup 195m/Hg owing to high-energy gamma radiation and longer half-life. Percentage breakthrough of /sup 195m/Hg was measured. The performance of the generator was assessed by determining the coefficient of variation of subsequent measurements

  5. Short-lived Isotopes from a Close-by AGB Star Triggering the Protosolar Nebula

    Science.gov (United States)

    Gallino, R.; Busso, M.; Wasserburg, G. J.; Straniero, O.

    The presence of short-lived isotopes in the early solar system, in particular 26Al, 41Ca, 60Fe, and 107Pd, point to a close-by and fresh nucleosynthesis source, possibly triggering the collapse of the protosolar nebula. We present the results of nucleosynthesis calculations based on an AGB polluting hypothesis. A general concordance of the predicted yields of the above radioactivities relative to 26Al can be obtained in the case of an intermediate mass AGB star with hot bottom burning in the envelope (thus producing 26Al), and mixing through a series of third dredge-up episodes a fraction of the C-rich and s-processed material from the He intershell with the extended envelope. Polution of the protosolar nebula with freshly synthesized material may derive from the efficient winds of the AGB star. In AGB stars, the s-process nucleosynthesis occurs both during the maximum phase of every thermal runaway, driven by the partial activation of the 22Ne(alpha,n)25Mg reaction, and in the interpulse phase, where the 13C nuclei are fully consumed in radiative conditions by the activation of the 13C(alpha,n)16O reaction. We have used different prescriptions for the amount of the 13C nuclei present in the intershell. A minimum amount of 13C is naturally expected in the ashes of H-shell burning. Possible formation of an extra "13C-pocket" derives from the injection of a small amount of protons from the envelope into the 12C-rich intershell during any third dredge-up episode, when the H-shell is inactivated. Prediction for other short-lived, 36Cl, 135Cs, and 205Pb, are given. General consequences for the pollution of the protosolar nebula with newly synthesized stable isotopes from the AGB winds are outlined. The origin of other detected short-lived nuclei, in particular 53Mn, 129I, and 182Hf, which cannot come from an AGB source, is analysed. The alternative trigger hypothesis by a close-by Supernova is discussed.

  6. Cancer incidence and risk in Alaskan natives exposed to radioactive fallout

    International Nuclear Information System (INIS)

    Stutzman, C.D.; Nelson, D.M.

    1986-01-01

    Cancer incidence in northern Alaskan villages exposed to radioactive fallout from nuclear weapons testing in the late 1950s and early 1960s was assessed using data from the Alaskan Native Tumor Registry. Previous studies have shown that cancer incidence in Alaskan natives differs from that in residents of the rest of the United States: rates of cancer of the nasopharynx and liver are higher in Alaskan native men and rates of cancer of the nasopharynx, gallbladder, cervix, and kidney are higher in Alaskan native women. Leukemia, breast cancer and bone sarcoma are the cancers most likely to result from fallout exposure in the Arctic, but the incidence of these cancers in the North Slope villages appeared to be lower than in either the entire Inuit population or the US population. The fallout radionuclides of potential health concern are cesium-137 and strontium-90, because of their abundance, long half-life, and chemical characteristics that facilitate transport through and concentration in the food chain and accumulation in sensitive tissues of the body. Radionuclide body burdens were determined in North Slope Inuit 25 years ago, because of their possible exposure to radioactive fallout via the lichen-caribou-man pathway. Cancer risk estimates have been calculated using highest average dose measurements from residents of Anaktuvuk Pass, under the assumption that peak exposure levels of the mid 1960s remained steady over the following 20 years. Worst-case estimates of expected cancer excess were calculated for leukemia, breast cancer and bone sarcoma

  7. Radiation doses and cancer risks in the Marshall Islands associated with exposure to radioactive fallout from Bikini and Enewetak nuclear weapons tests: summary.

    Science.gov (United States)

    Simon, Steven L; Bouville, André; Land, Charles E; Beck, Harold L

    2010-08-01

    for internal doses to the thyroid gland, external exposure was generally the major contributor to organ doses, particularly for red bone marrow and stomach wall. Internal doses to the stomach wall and red bone marrow were similar in magnitude, about 1 mGy to 7 mGy for permanent residents of the southern and mid-latitude atolls. However, adult residents of Utrik and Rongelap Island, which are part of the northern atolls, received much higher internal doses because of intakes of short-lived radionuclides leading to doses from 20 mGy to more than 500 mGy to red bone marrow and stomach wall. In general, internal doses to the colon wall were four to ten times greater than those to the red bone marrow and internal doses to the thyroid gland were 20 to 30 times greater than to the red bone marrow. Adult internal thyroid doses for the Utrik community and for the Rongelap Island community were about 760 mGy and 7,600 mGy, respectively. The highest doses were to the thyroid glands of young children exposed on Rongelap at the time of the Castle Bravo test of 1 March 1954 and were about three times higher than for adults. Internal doses from chronic intakes, related to residual activities of long-lived radionuclides in the environment, were, in general, low in comparison with acute exposure resulting from the intakes of radionuclides immediately or soon after the deposition of fallout. The annual doses and the population sizes at each atoll in each year were used to develop estimates of cancer risks for the permanent residents of all atolls that were inhabited during the testing period as well as for the Marshallese population groups that were relocated prior to the testing or after it had begun. About 170 excess cancers (radiation-related cases) are projected to occur among more than 25,000 Marshallese, half of whom were born before 1948. All but about 65 of those cancers are estimated to have already been expressed. The 170 excess cancers are in comparison to about 10

  8. Measurements of beta-decay half-lives of short-lived nuclei

    Energy Technology Data Exchange (ETDEWEB)

    Hirose, T.; Tsurita, Y.; Yamamoto, H.; Kawade, K. [Nagoya Univ. (Japan); Iida, T.; Takahashi, A.; Kasugai, Y.; Ikeda, Y.

    1997-03-01

    The {beta}-decay half-lives of short-lived nuclei produced by 14 MeV neutron bombardments were measured with Ge detectors, a High-rate spectroscopy amplifier (EG and G ORTEC model 973) and a Spectrum multi-scaler (Laboratory equipment corporation SMS-48) in the multi-scaling mode. The adequate corrections for pile-up and dead-time losses were made by applying source and pulser methods. The half-lives of {sup 53}V, {sup 53g}Fe, {sup 89m}Y and {sup 162}Tb were determined with uncertainties of 0.13-0.65%. It has been shown that previous values shorter than 10 min were systematically longer than the present ones. (author)

  9. Laser generation of proton beams for the production of short-lived positron emitting radioisotopes

    International Nuclear Information System (INIS)

    Spencer, I.; Ledingham, K.W.D.; Singhal, R.P.; McCanny, T.; McKenna, P.; Clark, E.L.; Krushelnick, K.; Zepf, M.; Beg, F.N.; Tatarakis, M.; Dangor, A.E.; Norreys, P.A.; Clarke, R.J.; Allott, R.M.; Ross, I.N.

    2001-01-01

    Protons of energies up to 37 MeV have been generated when ultra-intense lasers (up to 10 20 W cm -2 ) interact with hydrogen containing solid targets. These protons can be used to induce nuclear reactions in secondary targets to produce β + -emitting nuclei of relevance to the nuclear medicine community, namely 11 C and 13 N via (p, n) and (p,α) reactions. Activities of the order of 200 kBq have been measured from a single laser pulse interacting with a thin solid target. The possibility of using ultra-intense lasers to produce commercial amounts of short-lived positron emitting sources for positron emission tomography (PET) is discussed

  10. Radioactivity of radon and its short-lived decay products in room air, 2

    International Nuclear Information System (INIS)

    Shimo, Michikuni; Katoh, Takao

    1983-01-01

    In the reactor room of the Kyoto University Research Reactor Institute, the measurements of radon (Rn) and its short-lived decay products (Rn-Dts) were carried out under ventilated and non-ventilated conditions. The indoor activities were equal to outdoor ones under ventilated condition and those activities increased till about 10 times of outdoors under non-ventilated condition. We attempted to explain these results on a basis of a simple model. The calculations were performed taking into account: (1) supply of Rn and Rn-Dts from outdoor, (2) the emanation rate of Rn from the wall materials of building, (3) the removal rate of Rn-Dts by ventilation and wall deposition, and (4) the attachment rate of unattached atom to aerosols. In addition, natural ventilation were considered during periods without artificial ventilation. (author)

  11. New three-count technique for short-lived radon decay products in air

    International Nuclear Information System (INIS)

    Tian Deyuan; Lu Zhizhao

    1998-01-01

    Up to the present, radon and its short-lived decay products in air are usually monitored by means of a detection. But radon progeny, including RaB ( 214 Pb) and RaC ( 214 Bi) which are β and γ emitters, contribute about 90% to the equilibrium equivalent radon concentration (EECRn). Therefore, this paper introduces a new three-count technique by a β detector in the light of radioactive decay law and its boundary conditions during sampling and counting times to solve the Bateman equation. β (even low level β) instruments have been fairly popularized domestically and internationally. It can be used not only as an instrument for radon and its daughters in air, but also as a monitor for β airborne activity in the environment. This new method taps further the latent power of the present instrument and realizes various uses for a unit. (author)

  12. NMR detection of short-lived β-emitter {sup 12}N implanted in water

    Energy Technology Data Exchange (ETDEWEB)

    Sugihara, T., E-mail: sugihara@vg.phys.sci.osaka-u.ac.jp; Mihara, M.; Shimaya, J.; Matsuta, K.; Fukuda, M.; Ohno, J.; Tanaka, M.; Yamaoka, S.; Watanabe, K.; Iwakiri, S.; Yanagihara, R.; Tanaka, Y.; Du, H.; Onishi, K.; Kambayashi, S.; Minamisono, T. [Osaka University, Department of Physics (Japan); Nishimura, D. [Tokyo University of Science, Department of Physics (Japan); Izumikawa, T. [Niigata University, Radioisotope Center (Japan); Ozawa, A. [University of Tsukuba, Department of Physics (Japan); Ishibashi, Y. [RIKEN Nishina Center for Accelerator-Based Science (Japan); and others

    2017-11-15

    The beta-detected nuclear magnetic resonance (β-NMR) in liquid H{sub 2}O has been observed for the first time using a short-lived β-ray emitter {sup 12}N (I{sup π} = 1{sup +},T{sub 1/2}=11 ms). A nuclear spin polarized {sup 12}N beam with an energy of about 20 MeV/nucleon was implanted into an enclosed water sample. About 50 % of implanted {sup 12}N ions maintained nuclear polarization and exhibited a β-NMR spectrum. The chemical shift of {sup 12}N in H{sub 2}O relative to {sup 12}N in Pt was deduced to be −(3.6±0.5) × 10{sup 2} ppm.

  13. Dynamical Detection of Topological Phase Transitions in Short-Lived Atomic Systems

    Science.gov (United States)

    Setiawan, F.; Sengupta, K.; Spielman, I. B.; Sau, Jay D.

    2015-11-01

    We demonstrate that dynamical probes provide direct means of detecting the topological phase transition (TPT) between conventional and topological phases, which would otherwise be difficult to access because of loss or heating processes. We propose to avoid such heating by rapidly quenching in and out of the short-lived topological phase across the transition that supports gapless excitations. Following the quench, the distribution of excitations in the final conventional phase carries signatures of the TPT. We apply this strategy to study the TPT into a Majorana-carrying topological phase predicted in one-dimensional spin-orbit-coupled Fermi gases with attractive interactions. The resulting spin-resolved momentum distribution, computed by self-consistently solving the time-dependent Bogoliubov-de Gennes equations, exhibits Kibble-Zurek scaling and Stückelberg oscillations characteristic of the TPT. We discuss parameter regimes where the TPT is experimentally accessible.

  14. Separation efficiency of the MASHA facility for short-lived mercury isotopes

    Science.gov (United States)

    Rodin, A. M.; Belozerov, A. V.; Chernysheva, E. V.; Dmitriev, S. N.; Gulyaev, A. V.; Gulyaeva, A. V.; Itkis, M. G.; Kliman, J.; Kondratiev, N. A.; Krupa, L.; Novoselov, A. S.; Oganessian, Yu. Ts.; Podshibyakin, A. V.; Salamatin, V. S.; Siváček, I.; Stepantsov, S. V.; Vanin, D. V.; Vedeneev, V. Yu.; Yukhimchuk, S. A.; Granja, C.; Pospisil, S.

    2014-06-01

    The mass-separator MASHA built to identify Super Heavy Elements by their mass-to-charge ratios is described. The results of the off- and on-line measurements of its separation efficiency are presented. In the former case four calibrated leaks of noble gases were used. In the latter the efficiency was measured via 284 MeV Ar beam and with using the hot catcher. The ECR ion source was used in both cases. The -radioactive isotopes of mercury produced in the complete fusion reaction Ar+SmHg+xn were detected at the mass-separator focal plane. The half-lives and the separation efficiency for the short-lived mercury isotopes were measured. Potentialities of the MEDIPIX detector system have been demonstrated for future use at the mass-separator MASHA.

  15. The short-lived African turquoise killifish: an emerging experimental model for ageing.

    Science.gov (United States)

    Kim, Yumi; Nam, Hong Gil; Valenzano, Dario Riccardo

    2016-02-01

    Human ageing is a fundamental biological process that leads to functional decay, increased risk for various diseases and, ultimately, death. Some of the basic biological mechanisms underlying human ageing are shared with other organisms; thus, animal models have been invaluable in providing key mechanistic and molecular insights into the common bases of biological ageing. In this Review, we briefly summarise the major applications of the most commonly used model organisms adopted in ageing research and highlight their relevance in understanding human ageing. We compare the strengths and limitations of different model organisms and discuss in detail an emerging ageing model, the short-lived African turquoise killifish. We review the recent progress made in using the turquoise killifish to study the biology of ageing and discuss potential future applications of this promising animal model. © 2016. Published by The Company of Biologists Ltd.

  16. Production, study and use of short-lived nuclides in pure and applied nuclear research

    International Nuclear Information System (INIS)

    Bjoernstad, T.

    1986-01-01

    The thesis which is based on 17 published papers, reports on the on-line performance of the fast radiochemical separation system SISAK, technical devlopment in the preparation of sources for beta-particles and neutrons, and on important SISAK system improvements concerning liquid hold-up time. It further reports on the development of new production targets at ISOLDE for 600 MeV proton and 910 MeV 3 He-particle irradiations, on tests with a heavy ion beam of 1 GeV 12 C-particles, and on the present availability of mass-separated beams of the halogen elements through new ion source development. Some results from nuclear spectroscopic studies of nuclides in selected mass regions when using such new or improved techniques are given. Examples of techniques for practical application of short-lived nuclides in radiochemical analysis and for radiochemical production for medical purposes are presented

  17. Short-lived climate pollutant mitigation and the Sustainable Development Goals

    Science.gov (United States)

    Haines, Andy; Amann, Markus; Borgford-Parnell, Nathan; Leonard, Sunday; Kuylenstierna, Johan; Shindell, Drew

    2017-12-01

    The post-2015 development agenda is dominated by a set of Sustainable Development Goals (SDGs) that arose from the 2012 Rio+20 United Nations Conference on Sustainable Development. The 17 goals and 169 targets address diverse and intersecting aspects of human and environmental needs and challenges. Achieving the SDGs by 2030 requires implementing coordinated and concerted strategies and actions that minimize potential trade-offs and conflicts and maximize synergies to contribute to multiple SDGs. Measures to mitigate emissions of short-lived climate pollutants are an example of actions that contribute to multiple outcomes relevant to development. This Perspective highlights the interlinkages between these pollutants and the SDGs, and shows that implementing emissions reduction measures can contribute to achieving many of the SDGs.

  18. Behaviour of short-lived iodines in operating UO2 fuel elements

    International Nuclear Information System (INIS)

    Lipsett, J.J.; Hastings, I.J.; Hunt, C.E.L.

    1984-11-01

    Sweep gas experiments have been done to determine the behaviour of short-lived fission products within operating UO 2 fuel elements at linear powers of 45, 54, and 60 KW/m, and to burnups of 70, 80, and 50 MWh/kgU respectively. Although radioiodine transport was not observed directly during normal operation, equilibrium gap inventories for I-131 were deduced from the shutdown decay behaviour of the fission gases. These inventories were a strong function of fuel power and ranged from 10 GBq (0.27 Ci) to 100 GBq (2.7 Ci) over the range tested. We conclude that the iodine inventory was adsorbed onto the fuel and/or sheath surfaces with a volatile fraction of less than 10 -2 and a charcoal-filter-penetrating fraction of less than 2x10 -4

  19. Optimization of irradiation decay and counting times in nuclear activation analysis using short-lived nuclides

    International Nuclear Information System (INIS)

    Bjoernstad, T.

    This work describes a method and outlines a procedure for optim- ization of an activation analysis with respect to the experimental times, irradiation time, t(subi), decay time and counting time. The method is based on the 'minimum relative standard deviation criterion', and specially designed for the use on short-lived nuclides. A computer program, COMB1, is written in the BASIC language in order to make the calculations easier and faster. It is intended to be understandable, and easily applicable on a computer of modest size. Time and cost are important factors, especially for routine analysis on a service basis. In such cases one can often allow a controlled reduction in the analysis quality (through a higher relative standard deviation). The procedure outlined can therefore help find acceptable conditions by calculation of the 'best practical' (or reasonable) experimental time values, and the minimum number of accumulation cycles necessary to fulfil the requirements given. (Auth.)

  20. Simulation of radon short lived decay daughters' inhalation using the lung compartmental model

    International Nuclear Information System (INIS)

    Tomulescu, Vlad C.

    2002-01-01

    Radon and its short-lived decay daughters are the main source of radiation on natural ways for population. The radon gas, released from soil, water or construction materials is producing by radioactive decay the following solid daughters: Po-218, Bi-214, Pb-214, and Po-214, which can attach to aerosols, and consequently penetrate the organism by inhalation. The human respiratory tract can be approximated by aid of a compartment model that takes into account the different anatomical structures exposed to contamination and irradiation, as well as the respective physiological processes. This model is associated to a mathematical equation system that describes the behavior of the radioactive material inside the body. The results represent the dose equivalent on different organs and tissues, as a function of subject and the activity performed in contaminating environment. (author)

  1. Investigation of short-living fission products from the spontaneous fission of Cf-252

    International Nuclear Information System (INIS)

    Klonk, H.

    1976-01-01

    In this paper, a method of separating and measuring fission products of Cf-252 is presented. The measurement was achieved by means of γ-spectrometry and thus provides a quantitative analysis with a good separation of the fission products with respect to both atomic number Z and mass number A. The separation of the fission products from the fission source was achieved by means of solid traps. An automatic changing apparatus made it possible to keep irradiation and measuring times short, so even very short-lived fission products could be registered. The quantitative evaluation of primary fission products was made possible by correction according to Bateman equations. With that, the yields of single nuclides and the dispersion of charge can be determined. (orig./WL) [de

  2. Compton suppression spectrometry for analysis of short-lived neutron activation products in foods

    International Nuclear Information System (INIS)

    Anderson, D.L.; Cunningham, W.C.

    2008-01-01

    Compton suppression spectrometry was used to analyze foods for elements with short-lived neutron activation products (half-lives of about 2 minutes to 1.5 days). Analysis conditions were optimized to provide quality assurance analyses for iodine in FDA's Total Diet Study. Iodine mass fractions (0.075 to 2.03 mg/kg) were measured in 19 of 42 foods analyzed, with limits of detection (LODs) ranging from 0.03 to 1.4 mg/kg, mostly depending on NaCl content. LODs were lowered by up to a factor of 2 for 16 elements. Suppression factors ranged from about 2 to 8 over the energy range 400 to 3200 keV. (author)

  3. Magnetic moment of short lived {beta}-emitter {sup 24m}Al

    Energy Technology Data Exchange (ETDEWEB)

    Nishimura, D., E-mail: daiki@vg.phys.sci.osaka-u.ac.jp; Komurasaki, J.; Matsuta, K.; Mihara, M.; Matsumiya, R. [Osaka University, Department of Physics (Japan); Momota, S. [Kochi University of Technology (Japan); Ohtsubo, T. [Niigata University, Department of Physics (Japan); Izumikawa, T. [Niigata University, RI Center (Japan); Hirano, H. [Niigata University, Department of Physics (Japan); Kitagawa, A.; Kanazawa, M.; Torikoshi, M.; Sato, S. [National Institute of Radiological Sciences (Japan); Fukuda, M.; Ishikawa, D. [Osaka University, Department of Physics (Japan); Minamisono, T. [Fukui University of Technology (Japan); Watanabe, R.; Kubo, T. [Niigata University, Department of Physics (Japan); Nojiri, Y. [Kochi University of Technology (Japan); Alonso, J. R. [Lawrence Berkeley Laboratory (United States)

    2007-11-15

    The magnetic moment of short lived {beta}-emitter {sup 24m}Al (426 keV, I{sup {pi}} = 1{sup +}, T{sub 1/2} = 131 ms) has been measured by means of {beta}-NMR technique, for the first time. From the {beta}-NMR spectrum, the magnetic moment was determined as |{mu}({sup 24m}Al)|=(2.99{+-}0.09){mu}{sub N}. Combined with the known magnetic moment of the mirror partner {sup 24m}Na, the expectation value of < S{sub z} > is obtained to be (0.08 {+-} 0.12). These values are reproduced well by the shell model calculation.

  4. Radiotracer diffusion in semiconductors and metallic compounds using short-lived isotopes

    CERN Multimedia

    Deicher, M; Kronenberg, J; Wagner, F E

    The transport of atoms in solids is of central importance for solid state physics, chemistry, metallurgy, and material sciences. Since the mobility of atoms in solids contributes to many physical phenomena the study of diffusion processes is of fundamental interest for solid state physics. Diffusion processes were frequently investigated using radioactive isotopes (radiotracers). The application of short-lived isotopes delivered at ISOLDE extends substantially the possibilities of investigating diffusion processes in solids. In particular, a new experimental set-up to be installed at ISOLDE in this year will enable the use of radioactive isotopes with half-lives down to minutes. Alternatively, in special cases diffusion processes can be investigated with help of hyperfine techniques on an atomic scale, like by perturbed $\\gamma \\gamma$-angular correlation (PAC). Here, the motion of the atom of interest becomes visible directly via characteristic changes in the measured PAC spectra.

  5. Reconstruction and analysis of cesium-137 fallout deposition patterns in the Marshall Islands

    Science.gov (United States)

    Whitcomb, Robert Cleckley, Jr.

    Estimates of 137Cs deposition due to fallout originating from nuclear weapons testing in the Marshall Islands have been made for several locations in the Marshall Islands. These retrospective estimates were based primarily on historical exposure rate and gummed film measurements. The methods used to reconstruct these deposition estimates are specific for six of the Pacific tests. These methods are also similar to those used in the National Cancer Institute study for reconstructing 131I deposition from the Nevada Test Site. Reconstructed cumulative deposition estimates are validated against contemporary measurements of 137Cs concentration in soil. This validation work also includes an accounting for estimated global fallout contributions. These validations show that the overall geometric bias in predicted-to-observed (P/O) ratios is 1.0 (indicating excellent agreement). The 5th and 95th percentile range of this distribution is 0.35--2.95. The P/O ratios for estimates using historical gummed film measurements tend to slightly over-predict more than estimates using exposure rate measurements. The methods produce reasonable estimates of deposition confirming that radioactive fallout occurred at atolls further south of the four northern atolls recognized by the Department of Energy as being affected by fallout. The deposition estimate methods, supported by the very good agreement between estimates and measurements, suggest that these methods can be used for other weapons testing fallout radionuclides with confidence.

  6. CARIBIC observations of short-lived halocarbons and carbonyl sulphide over Asia

    Science.gov (United States)

    Leedham, E.; Wisher, A.; Oram, D.; Baker, A. K.; Brenninkmeijer, C. A.

    2013-12-01

    The CARIBIC project (Civil Aircraft for the Regular Investigation of the atmosphere Based on an Instrument Container, www.caribic-atmospheric.com) aims to investigate the spatial and temporal distribution of a wide-range of compounds, including those of marine origin/influence, via ~monthly flights to collect in situ data and whole air samples aboard a commercial Lufthansa aircraft. CARIBIC measures up to an altitude of 12 km, allowing the influence of marine compounds on the upper troposphere/lower stratosphere (UTLS) to be explored. In particular, CARIBIC is a useful tool for exploring the impact of very short lived halocarbons (e.g. CH2Br2, CHBr3), whose impact on stratospheric ozone is dependent on convective uplift to the UTLS, a process which is not yet fully quantified. As part of the suite of CARIBIC measurements, whole air samples are analysed at the University of East Anglia (UEA) via gas chromatography mass spectrometry for carbonyl sulphide (OCS) and up to 40 halocarbons (accounting for virtually 100% of organic chlorine, bromine and iodine in the UTLS). Here we present an overview of short-lived halocarbons and OCS measured by CARIBIC. We focus on two regions of particular interest. (1) measurements made in 2012 over the tropical west Pacific to link with UEA measurements made during the SHIVA campaign. (2) measurements made during a collection of flights over India in 2008. Flights over India investigated the impact of monsoon circulation on the distribution of these compounds; for example, elevated concentrations of OCS were seen in CARIBIC samples taken over India during the summer monsoon (July - September). These flights, along with a wider range of flights over Asia (from Frankfurt to Guangzhou, Manila, Bangkok and Kuala Lumpur) can provide unique information on the influence of tropical convection and monsoon circulation on halocarbon and OCS transport within this region.

  7. Evaluation of regional pulmonary function using short-lived radioactive gases

    Energy Technology Data Exchange (ETDEWEB)

    Ashitaka, Tsuyoshi [Toho Univ., Tokyo (Japan). School of Medicine

    1993-05-01

    We investigated the application of short-lived radioactive gases for the assessment of regional pulmonary function, particularly diffusing capacity, in patients with chronic obstructive lung disease and interstitial lung disease. Short-lived radioactive gases including C[sup 15]O-O, [sup 11]CO[sub 2], and [sup 11]CO were produced using a baby cyclotron for medical care. Using a [gamma] camera, breath-holding images were taken serially after inhalation of the radioactive gases. The first exponential component of time-activity curve was analyzed to obtain clearance rate, which was expressed as exponential coefficient ([lambda]). Moreover, we created a functional map which was calculated by the clearance rate of [sup 11]CO[sub 2] as a percentage. Regional clearance rates of each gas in normal volunteers revealed higher values in the lower lung field than in the upper lung field. Whole lung clearance rates ([lambda]) of each gas in patients correlated well with D[sub LCO]/V[sub A], which indicates diffusing capacity. The functional map showed decreased regional diffusion closely matched to the perfusion defects seen by [sup 99m]Tc-MAA perfusion images. However, in certain interstitial lung diseases decreased clearance of [sup 11]CO[sub 2] was observed in regions having no evidence of perfusion defects. We concluded the functional map display of [sup 11]CO[sub 2] is useful indicator of the regional diffusing capacity of both the normal and diseased lung, and that it is beneficial to analyze the pathogenic physiology of diseased lungs by making a comparison between the functional map of [sup 11]CO[sub 2] and [sup 99m]Tc-MAA perfusion images. (author).

  8. Antigen modulation of the immune response. III. Evaluation of the hypothetical short-lived memory cell

    International Nuclear Information System (INIS)

    Feldbush, T.L.; Lande, I.; Bryan, B.; O'Neill, E.

    1974-01-01

    The putative short-lived memory cells, whose existence has been suggested by the results of secondary adoptive transfer experiments, were investigated. On the basis of the following evidences we have concluded that the short-lived memory cell is probably an artifact of the adoptive transfer technique: when immune thoracic duct lymphocytes, known to consist predominantly of long-lived memory cells, were transferred to irradiated recipients and challenged at various times after transfer, approximately 80 to 90 percent of the initial response was absent by Day 14 challenge; preirradiating adoptive recipients with increasing dose of x-irradiation tended to lengthen the observed half life of memory cells; single or multiple treatments of immune donors with 0.3 mg Vinblastin before transfer resulted in neither a depression of the initial secondary response nor an alteration in the rate of decline of the memory potential; reconstitution of irradiated hosts with normal spleen cells one day before transfer of memory cells and challenge resulted in inhibition of the adoptive secondary response; and the transfer of memory cells to antigen free intermediate hosts, in which they were allowed to reside for one day or fourteen days before transfer to irradiated recipients, resulted in only a slight decline in their capacity to respond. We propose that the rapid decline of memory potential in adoptive recipients challenged at various times after transfer is due to modulating effects by the hosts as it recovers from irradiation. These effects may be the result of cell crowding or the loss of irradiation-produced stimulatory factors. The relevance of these findings to adoptive transfer systems in general and the secondary response of intact animals is discussed

  9. Muscle senescence in short-lived wild mammals, the soricine shrews Blarina brevicauda and Sorex palustris.

    Science.gov (United States)

    Hindle, Allyson G; Lawler, John M; Campbell, Kevin L; Horning, Markus

    2009-06-01

    Red-toothed (soricine) shrews are consummate predators exhibiting the highest energy turnovers and shortest life spans (ca. 18 months) of any mammal, yet virtually nothing is known regarding their physiological aging. We assessed the emerging pattern of skeletal muscle senescence (contractile/connective tissue components) in sympatric species, the semi-aquatic water shrew (WS), Sorex palustris, and the terrestrial short-tailed shrew (STS), Blarina brevicauda, to determine if muscle aging occurs in wild, short-lived mammals (H(0): shrews do not survive to an age where senescence occurs), and if so, whether these alterations are species-specific. Gracilis muscles were collected from first-year (n=17) and second-year (n=17) field-caught shrews. Consistent with typical mammalian aging, collagen content (% area) increased with age in both species (S. palustris: approximately 50%; B. brevicauda: approximately 60%). Muscle was dominated by stiffer Type I collagen, and the ratio of collagen Type I:Type III more than doubled with age. The area ratio of muscle:collagen decreased with age in both species, but was considerably lower in adult STS, suggesting species-specificity of senescence. Extracellular space was age-elevated in B. brevicauda, but was preserved in S. palustris ( approximately 50 vs. 10% elevation). Though juvenile interspecific comparisons revealed no significance, adult WS myocytes had 68% larger cross-sectional area and occurred at 28% lower fibers/area than those of adult STS. We demonstrate that age-related muscle senescence does occur in wild-caught, short-lived mammals, and we therefore reject this classic aging theory tenet. Our findings moreover illustrate that differential age adjustments in contractile/connective tissue components of muscle occur in the two species of wild-caught shrews. (c) 2009 Wiley-Liss, Inc.

  10. Muscle Senescence in Short-Lived Wild Mammals, the Soricine Shrews Blarina brevicauda and Sorex palustris

    Science.gov (United States)

    HINDLE, ALLYSON G.; LAWLER, JOHN M.; CAMPBELL, KEVIN L.; HORNING, MARKUS

    2015-01-01

    Red-toothed (soricine) shrews are consummate predators exhibiting the highest energy turnovers and shortest life spans (ca. 18 months) of any mammal, yet virtually nothing is known regarding their physiological aging. We assessed the emerging pattern of skeletal muscle senescence (contractile/connective tissue components) in sympatric species, the semi-aquatic water shrew (WS), Sorex palustris, and the terrestrial short-tailed shrew (STS), Blarina brevicauda, to determine if muscle aging occurs in wild, short-lived mammals (H0: shrews do not survive to an age where senescence occurs), and if so, whether these alterations are species-specific. Gracilis muscles were collected from first-year (n = 17) and second-year (n = 17) field-caught shrews. Consistent with typical mammalian aging, collagen content (% area) increased with age in both species (S. palustris: ~50%; B. brevicauda: ~60%). Muscle was dominated by stiffer Type I collagen, and the ratio of collagen Type I:Type III more than doubled with age. The area ratio of muscle:collagen decreased with age in both species, but was considerably lower in adult STS, suggesting species-specificity of senescence. Extracellular space was age-elevated in B. brevicauda, but was preserved in S. palustris (~50 vs. 10% elevation). Though juvenile interspecific comparisons revealed no significance, adult WS myocytes had 68% larger cross-sectional area and occurred at 28% lower fibers/area than those of adult STS. We demonstrate that age-related muscle senescence does occur in wild-caught, short-lived mammals, and we therefore reject this classic aging theory tenet. Our findings moreover illustrate that differential age adjustments in contractile/connective tissue components of muscle occur in the two species of wild-caught shrews. PMID:19296507

  11. DEMOGRAPHY OF ALPINE SHORT-LIVED PLANTS, LONGEVITY AND ONTOGENY STAGE DURATIONS

    Directory of Open Access Journals (Sweden)

    E. S. Kazantseva

    2016-01-01

    Full Text Available The aim - to evaluate lifespan (full cycle and ontogeny stage durations of nine alpine short-lived North- West Caucasus plants.Methods. For calculation we used a new method which was developed and suggested earlier by us. This method is based on a discrete ontogeny description and on the probability theory and random processes. The data on the monitoring of the marked individuals were collected during six years.Results. We found out that the lifespan of Anthyllis vulneraria is 2.6±0.3 years (hereinafter “±” is Standard error, Draba hispida – 4.5±0.3, Murbeckiella huetii – 4.6±1.1, Carum meifolium – 7.8±1.4, Eritrichium caucasicum – 9.1±1.4, Trifolium badium – 10.3±2.6, Sedum tenellum – 11±2.05, Androsace albana – 12.1±2.5, Minuartia recurva – 22.9±4.5. Also we demonstrated the matrix population models for studied plants, which show the probability of transition of individuals from one ontogeny stage to another in time interval (in our experiment – 1 year.Conclusion. Mortality of seedlings and juvenile plants, except Murbeckiella huetii, is around and more than 50%. Two years is the minimal amount of time that is necessary for full cycle of short-lived alpine plants, as it was shown for Anthyllis vulneraria, Murbeckiella huetii и Trifolium badium. A 3-12 years lifespan was calculated for other studied species. Persistence of Eritrichium caucasicum and Androsace albana populations provided by resistance of adult vegetative plants.

  12. Proficiency testing for radionuclides

    International Nuclear Information System (INIS)

    Faanhof, A.; Kotze, O.; Louw, I.

    2010-01-01

    Proficiency testing in general is only useful when it suites a certain purpose. With regards to radionuclides basically three fields of interest can be identified: (I)Foodstuffs-Introduced in the early 1960's to monitor the fall-out of nuclear tests and eventually the pathway to foodstuffs fit for human consumption. The demand for analysis increased substantially after the Chernobyl accident. (II) Natural radioactivity-Associated with mining and mineral processing of uranium and thorium baring mineral resources throughout the world where the radionuclides from the natural uranium and thorium decay series are found to pose concern for professional and public exposure. (III) Artificial radioactivity-This category covers mostly the long-lived nuclides generated by nuclear fission of the fuel used in nuclear power plants, research reactors and nuclear bomb tests. All three categories require a specific approach for laboratories to test their ability to analyze specific radio nuclides of interest in a variety of matrices. In this lecture I will give a compiled overview of the required radioanalytical skills, analysis sensitivity needed and radionuclides of interest, with more specific emphasis on QAQC of water sources and the recommended monitoring approach. And provide information on available reference materials and organizations/institutes that provide regular exercises for participating laboratories. I will also briefly communicate on the advantages and disadvantages of ISO/IEC 17025 accreditation for test laboratories, which is these days a prerequisite in national and international trade especially where foodstuffs and mineral products are concerned.

  13. A fall-out shelter

    International Nuclear Information System (INIS)

    Blatchford, J.M.A.

    1982-01-01

    A strong structure of precast concrete for use as, for example, a fallout shelter, strong-room or electricity sub-station is described. The major portion is generally tubular in construction and rectangular in cross-section. The tube may be formed in one piece or with two directed channel elements. Pairs of U legs abut either along the sides or along the top and bottom. End slabs close the compartment. An entrance shaft is formed by an upstanding channel element with upper and lower end slabs; alternatively the entrance shaft may be horizontal. Doors or hatches are provided. The whole structure may be buried. This invention provides a structure capable of withstanding considerable overpressure and of offering good resistance to radiation and is cheap and simple to manufacture. (U.K.)

  14. Radionuclide production for PET with a linear electrostatic accelerator

    International Nuclear Information System (INIS)

    Shefer, R.E.; Hughey, B.J.; Klinkowstein, R.E.; Welch, M.J.

    1993-01-01

    A new type of linear electrostatic accelerator for the production of short-lived radionuclides for PET has been developed at Science Research Laboratory. The tandem cascade accelerator (TCA) is a low energy (3.7 MeV) proton and deuteron accelerator which can generate the four short-lived PET radionuclides in the quantities required for clinical use. The compact size, low weight, low power consumption and reduced radiation shielding requirements of the TCA result in a significant reduction in capital and operating costs when compared with higher energy cyclotron-based systems. Radioisotope target for the production of O-15, F-18, N-13 and C-11 have been designed specifically for use with the low energy TCA beam. A simple to use PC-based computer control system allows fully automated system operation and advanced scheduling of isotope production. Operating experience with the TCA and its PET radionuclide targets is described

  15. The combined effect of two different bone-seeking radionuclides on the induction of osteosarcomas in mice

    International Nuclear Information System (INIS)

    Mueller, W.A.; Luz, A.; Linzner, U.; Murray, A.B.

    1991-01-01

    The effect of injection of 1.85kBq/kg of the long-lived radionuclide 227 Ac on the induction of osteosarcomas in female NMRI-mice by different dose levels of the short-lived radionuclide 227 Th (18.5, 74, and 185 kBq/kg), of the short-lived radionuclide 224 Ra (18.5 kBq/kg and 185 kBq/kg) and of the short-lived β-emitter 177 Lu (100 MBq/kg and 200 MBq/kg) was investigated. The results showed in all cases that combined incorporation of two radionuclides at the levels of radioactivity studied has a lower biological effect than the sum of the effects of the components administered singly. (author)

  16. Lichens of the alps as biomonitors for radioactive fallout

    International Nuclear Information System (INIS)

    Hofmann, W.; Gastberger, M.; Tuerk, R.

    1995-07-01

    time ago. Due to various reasons the initial contamination patterns of lichens can slowly be altered. In the case of this study the contamination deposited in the soil per unit surface area does not show significant differences between the sampling locations. On the other hand the activities per unit lichen dry weight differ significantly between some sampling locations. This can partly be caused by different growth rates of the lichens. Furthermore, lichens were not only contaminated directly by the Chernobyl fallout, but they may also have absorbed radionuclides from the soil after the initial exposure. For all the examined Cetraria islandica samples the average uptake can be estimated with 20 % to 40 % of the total 137 Cs. In general, the influence of these uncertainties increases with increasing time between contamination and sampling. In conclusion lichens can still be used as biomonitors of the radioactive contamination a few years after a fallout has occurred, but additional uncertainties have to be considered. Hence only lichens from sites with similar growth conditions should be compared. (author)

  17. Fallout 137Cs in reindeer herders in Arctic Norway.

    Science.gov (United States)

    Skuterud, Lavrans; Thørring, Håvard

    2015-03-03

    Reindeer herders in the Arctic were among the most heavily exposed populations to the global fallout from nuclear weapons testing in the 1950s and 1960s, due to high transfer of radionuclides in the lichens-reindeer-human food chain. Annual studies of (137)Cs in reindeer herders in Kautokeino, Norway, were initiated in 1965 to monitor radiation doses and follow environmental (137)Cs behavior. The (137)Cs concentrations declined from the peak in 1965 with effective half-times of 6-8 years, only interrupted by a temporary doubling in levels from 1986 to 1987 due to the Chernobyl fallout. During the period of 1950-2010 an average herder received an integrated effective dose from incorporated (137)Cs of about 18 mSv. This dose represents an insignificant increase in the risk for developing cancer. Health studies even show a significantly lower cancer incidence among Sámis and reindeer herders in northern Norway compared to other populations in the same area.

  18. Variation in the local population dynamics of the short-lived Opuntia macrorhiza (Cactaceae).

    Science.gov (United States)

    Haridas, C V; Keeler, Kathleen H; Tenhumberg, Brigitte

    2015-03-01

    Spatiotemporal variation in demographic rates can have profound effects for population persistence, especially for dispersal-limited species living in fragmented landscapes. Long-term studies of plants in such habitats help with understanding the impacts of fragmentation on population persistence but such studies are rare. In this work, we reanalyzed demographic data from seven years of the short-lived cactus Opuntia macrorhiza var. macrorhiza at five plots in Boulder, Colorado. Previous work combining data from all years and all plots predicted a stable population (deterministic log lamda approximately 0). This approach assumed that all five plots were part of a single population. Since the plots were located in a suburban-agricultural interface separated by highways, grazing lands, and other barriers, and O. macrorhiza is likely dispersal limited, we analyzed the dynamics of each plot separately using stochastic matrix models assuming each plot represented a separate population. We found that the stochastic population growth rate log lamdaS varied widely between populations (log lamdaS = 0.1497, 0.0774, -0.0230, -0.2576, -0.4989). The three populations with the highest growth rates were located close together in space, while the two most isolated populations had the lowest growth rates suggesting that dispersal between populations is critical for the population viability of O. macrorhiza. With one exception, both our prospective (stochastic elasticity) and retrospective (stochastic life table response experiments) analysis suggested that means of stasis and growth, especially of smaller plants, were most important for population growth rate. This is surprising because recruitment is typically the most important vital rate in a short-lived species such as O. macrorhiza. We found that elasticity to the variance was mostly negligible, suggesting that O. macrorhiza populations are buffered against large temporal variation. Finally, single-year elasticities to means

  19. Harvard-MIT research program in short-lived radiopharmaceuticals. Technical progress report, 1991

    Energy Technology Data Exchange (ETDEWEB)

    Adelstein, S.J.

    1991-12-31

    This report presents research on radiopharmaceuticals. The following topics are discussed: antibody labeling with positron-emitting radionuclides; antibody modification for radioimmune imaging; labeling antibodies; evaluation of technetium acetlyacetonates as potential cerebral blood flow agents; and studies in technetium chemistry. (CBS)

  20. Practical Applications of Short-Lived Radionuclides in Activation Analysis; Applications Pratiques des Radioelements de Courte Periode dans l'Analyse par Activation; ПРАКТИЧЕСКОЕ ПРИМЕНЕНИЕ КОРОТКОЖИВУЩИХ РАДИОИЗОТОПОВ ПРИ АКТИВАЦИОННОМ АНАЛИЗЕ; Aplicaciones Practicas de los Radionuclidos de Periodo Corto en el Anausis por Activacion

    Energy Technology Data Exchange (ETDEWEB)

    Chinaglia, B. Chin; Ciuffolotti, L.; Fasolo, G. B.; Malvano, R. [Centre de Recherches Nucleaires Sorin, Saluggia (Italy)

    1963-03-15

    Activation analysis by means of short-lived radionuclides has found some remarkable applications in the SORIN Research Centre at Saluggia. The paper describes the special techniques of irradiation, chemical separation and measurement required to obtain adequate accuracy and good sensitivity. It has proved possible to apply the method to analysis of elements with a half-life down to 10 s, with a consequent enormous gain in time. The method has been of benefit in several different spheres, as in solving metallurgical and technical problems (e.g. study of impurities in special-purpose materials) and in geochemistry and biology. (author) [French] L'analyse par activation au moyen de radioelements de courte periode a trouve de remarquables applications au Centre de recherches SORIN, a Saluggia. On decrit dans le memoire les techniques particulieres d'irradiation, de separation chimique et de mesure qui sont indispensables pour obtenir une precision satisfaisante ainsi qu'une bonne sensibilite. On a pu ainsi etendre la methode a l'analyse dfelements dont la periode peut atteindre dix secondes, realisant de cette facon un remarquable gain de temps. Plusieurs branches ont tire profit de cette methode, soit dans la resolution de problemes metallurgiques et technologiques (par exemple etude des impuretes dans des materiaux d'emploi special), soit en geochimie et en biologie. (author) [Spanish] El analisis por activacion empleando radionuclidos de periodo corto ha encontrado aplicaciones notables en el Centro de Investigaciones SORIN de Saluggia. En la memoria se describen tecnicas especiales de irradiacion, de separacion quimica y de medicion, indispensables para alcanzar una precision y sensibilidad satisfactorias. Se han podido analizar elementos de un periodo de hasta 10 s, logrando asi un considerable ahorro de tiempo. El metodo ha beneficiado a muchos campos de aplicacion, sea para resolver problemas de metalurgia y technologia (por ejemplo en el estudio de las

  1. Tracking Radioactive Fallout from the Fukushima Dai-ichi Accident in Arctic Snow

    Science.gov (United States)

    Osterberg, E. C.; Thompson, J.; Landis, J.; Albert, M. R.; Campbell, S. W.; Hawley, R. L.; Virginia, R. A.

    2011-12-01

    The March 11, 2011 magnitude 9.0 Tohoku, Japan earthquake produced a tsunami that inundated the Fukushima Dai-ichi nuclear power plant and led to the accidental release of radioactive 131I, 132Te, 134Cs, and 137Cs to the atmosphere. The Japanese Nuclear Safety Commission estimates that 12,000 TBq of 137Cs were released to the atmosphere during the incident, which represents ~14% of the total estimated 137Cs emission from the Chernobyl disaster in April 1986. Measurements of airborne radiation collected at the Fukushima plant illustrate that >50% of the total emitted radiation was released on March 15 and 16 associated with explosions and fires at reactor units 1, 2, and 4, and 70% was emitted in the first 5 days of the event. The source of the radiation is thus well constrained in time and space, providing an opportunity to better understand long-range atmospheric transport processes from Asia to the Arctic, while also assessing the magnitude of the fallout in the Arctic. Here we describe the 137Cs and 134Cs fallout flux near Thule, Greenland (1700 m a.s.l.), at Summit (3200 m a.s.l.), Greenland, and within Denali National Park, Alaska (2400-3900 m a.s.l.) based on series of large-volume (5-15 l) snow pit samples collected in June and July, 2011. In addition to assessing the spatial variability of Fukushima fallout in the Arctic, the elevation range of samples allows for an analysis of any vertical heterogeneity in fallout transport and deposition. Major ion concentrations and stable water isotope ratios are used to confirm the seasonal timing of the Fukushima fallout horizon in the snowpack. Radiocesium was concentrated and isolated from the snow pit meltwater using the well-established ammonium phosphomolybdate (AMP) adsorption method, and 134Cs and 137Cs concentrations were measured using gamma spectrometry with a Canberra 3523 well-type intrinsic Ge-detector at the Dartmouth College Short-Lived Isotope Laboratory. NOAA HYPLIT atmospheric forward

  2. Automating the Coupling of ORIGEN with GADRAS via the Fallout Analysis Tool for National Technical Nuclear Forensics

    International Nuclear Information System (INIS)

    Monterial, Mateusz; Jodoin, Vincent J.; Lefebvre, Jordan P.; Peplow, Douglas E.; Hooper, David A.

    2012-01-01

    Nuclear forensic teams will be deployed to collect and evaluate fallout samples on the ground in the scenario of a low-yield nuclear detonation in a heavily populated area. Quick non-destructive methods of predicting the quality of the sample before it is analyzed in detail are essential for efficient post-event collections. In this work, the process of exporting Defense Land Fallout Interpretive Code (DELFIC) results into Gamma Detector Response and Analysis Software (GADRAS) has been automated within the Fallout Analysis Tool. This coupling allows for the simulation of detector responses to fallout samples with varying degrees of fractionation. The degree to which the samples are fractionated depends on the location of the samples in the fallout field. In the following study, this phenomenon is examined, as its understanding is important to the investigation of debris distribution. The simulated detector spectra from GADRAS can be used to compare peak ratios of volatile-refractory isotope pairs in order to determine the degree of fractionation. Simulated fractionated fallout samples from DELFIC for a 10 kt, pure 235U fission surface burst were modeled for distances ranging to 256 km out from ground zero, and for times up to 1 week from detonation. The fractionation ratios, also known as r values, from isotope concentrations, photon lines and peak areas of four volatile-refractory pairs were calculated and compared. Fractionation prediction via the peak areas method was evaluated for each pair by comparing the results with the simulated radionuclide inventory.

  3. Determination of copper in biological materials by neutron activation analysis using short-lived 66Cu

    International Nuclear Information System (INIS)

    Dybczynski, R.; Danko, B.; Kaczorowski, J.

    1989-01-01

    A method for determination of copper traces in biological materials based on neutron activation employing 65 Cu(n, γ) 66 Cu reaction and preconcentration by extraction chromatography has been devised. The 200-500 mg samples after wet digestion and evaporation were dissolved in glycine solution and after pH adjusting to ca. 4.4 were passed through the column with Lix 64N on Bio Beads SM-1 for isolation of copper traces from the matrix elements. Other cations were selectively eluted with 0.1 mol x 1 -1 (glycine-HNO 3 ) buffer, 1 mol x 1 -1 in NH 4 NO 3 (pH = 3.6). The resin bed with quantitatively retained copper was sealed in the PE bag and irradiated together with Cu standards in EWA reactor using pneumatic tube facility. The activity of the short-lived 66 Cu was measured in samples and standard by gamma-ray spectrometry with Ge(Li) detector. Good accuracy of the method was confirmed by analysis of the following certified reference materials: NBS 1571 Orchad leaves, IAEA H-4 Animal muscle, IAEA V-8 Rye flour, IAEA A-11 milk powder. The detection limit amounted to 0.34 mg/kg, for the sample weight of 500 mg. (author)

  4. Quantitative cerebral blood flow patterns with the short lived isotope 195m Au

    International Nuclear Information System (INIS)

    Lindner, P.; Nickel, O.

    1984-01-01

    A previously reported theory for quantitative cerebral blood flow measurements using intravenously injected nondiffusible radiotracers has been applied on patients after stroke and on volunteers undergoing a mental stimulation exercise. Quantitative measurements of cerebral blood flow patterns (in ml/min/100g) not only in p.a. but also in lateral views of the brain are possible by using of the short-lived (30 sec) isotope Au 195m. The energy spectrum of the eluate of the generator shows two strong photon peaks, one at 68 keV and a second at 262 keV. The 68 keV peak is suitable for perfusion studies in lateral views of the hemispheres, no 'look through' effect is seen. The 262 keV peak is good for studies in p.a. positions. The studies last less than 1 minute and can be repeated after 3 minutes. Parametric images for quantitative regional cerebral blood flow can be generated. The area of occluded vessels in the case of stroke can be made visible. Quantitative activation patterns of cerebral blood flow during mental stimulation can be generated. After optical stimulation a clear increase of blood flow was seen in the visual cortex. The results prove that not only with freely diffusible (like Xenon) but also with nondiffusible indicators like 195m Au it is possible to measure quantitatively cerebral blood flow patterns. Au 195m is very advantageous for quantitative clinical investigations of cerebrovascular disease. (Author)

  5. ''Sleeping reactor'' irradiations: Shutdown reactor determination of short-lived activation products

    International Nuclear Information System (INIS)

    Jerde, E.A.; Glasgow, D.C.

    1998-01-01

    At the High-Flux Isotope Reactor (HFIR) at the Oak Ridge National Laboratory, the principal irradiation system has a thermal neutron flux (φ) of ∼ 4 x 10 14 n/cm 2 · s, permitting the detection of elements via irradiation of 60 s or less. Irradiations of 6 or 7 s are acceptable for detection of elements with half-lives of as little as 30 min. However, important elements such as Al, Mg, Ti, and V have half-lives of only a few minutes. At HFIR, these can be determined with irradiation times of ∼ 6 s, but the requirement of immediate counting leads to increased exposure to the high activity produced by irradiation in the high flux. In addition, pneumatic system timing uncertainties (about ± 0.5 s) make irradiations of 9 Be(γ,n) 8 Be, the gamma rays principally originating in the spent fuel. Upon reactor SCRAM, the flux drops to ∼ 1 x 10 10 n/cm 2 · s within 1 h. By the time the fuel elements are removed, the flux has dropped to ∼ 6 x 10 8 . Such fluxes are ideal for the determination of short-lived elements such as Al, Ti, Mg, and V. An important feature of the sleeping reactor is a flux that is not constant

  6. Short-Lived Buildings in China: Impacts on Water, Energy, and Carbon Emissions.

    Science.gov (United States)

    Cai, Wenjia; Wan, Liyang; Jiang, Yongkai; Wang, Can; Lin, Lishen

    2015-12-15

    This paper has changed the vague understanding that "the short-lived buildings have huge environmental footprints (EF)" into a concrete one. By estimating the annual floor space of buildings demolished and calibrating the average building lifetime in China, this paper compared the EF under various assumptive extended buildings' lifetime scenarios based on time-series environmental-extended input-output model. Results show that if the average buildings' lifetime in China can be extended from the current 23.2 years to their designed life expectancy, 50 years, in 2011, China can reduce 5.8 Gt of water withdrawal, 127.1 Mtce of energy consumption, and 426.0 Mt of carbon emissions, each of which is equivalent to the corresponding annual EF of Belgium, Mexico, and Italy. These findings will urge China to extend the lifetime of existing and new buildings, in order to reduce the EF from further urbanization. This paper also verifies that the lifetime of a product or the replacement rate of a sector is a very important factor that influences the cumulative EF. When making policies to reduce the EF, adjusting people's behaviors to extend the lifetime of products or reduce the replacement rate of sectors may be a very simple and cost-effective option.

  7. New use of global warming potentials to compare cumulative and short-lived climate pollutants

    Science.gov (United States)

    Allen, Myles R.; Fuglestvedt, Jan S.; Shine, Keith P.; Reisinger, Andy; Pierrehumbert, Raymond T.; Forster, Piers M.

    2016-08-01

    Parties to the United Nations Framework Convention on Climate Change (UNFCCC) have requested guidance on common greenhouse gas metrics in accounting for Nationally determined contributions (NDCs) to emission reductions. Metric choice can affect the relative emphasis placed on reductions of `cumulative climate pollutants' such as carbon dioxide versus `short-lived climate pollutants' (SLCPs), including methane and black carbon. Here we show that the widely used 100-year global warming potential (GWP100) effectively measures the relative impact of both cumulative pollutants and SLCPs on realized warming 20-40 years after the time of emission. If the overall goal of climate policy is to limit peak warming, GWP100 therefore overstates the importance of current SLCP emissions unless stringent and immediate reductions of all climate pollutants result in temperatures nearing their peak soon after mid-century, which may be necessary to limit warming to ``well below 2 °C'' (ref. ). The GWP100 can be used to approximately equate a one-off pulse emission of a cumulative pollutant and an indefinitely sustained change in the rate of emission of an SLCP. The climate implications of traditional CO2-equivalent targets are ambiguous unless contributions from cumulative pollutants and SLCPs are specified separately.

  8. Emission channeling with short-lived isotopes lattice location of impurities in semiconductors and oxides

    CERN Multimedia

    We propose to perform emission channeling lattice location experiments in a number of semiconductor and oxide systems of technological relevance: \\\\- The lattice location of the transition metal probes $^{56}$Mn ($\\textit{t}_{1/2}$=2.6 h), $^{59}$Fe (45 d), $^{61}$Co (1.6 h) and $^{65}$Ni (2.5 h) is to be investigated in materials of interest as dilute magnetic semiconductors, such as GaMnAs, GaMnN, GaFeN, AlGaN, SiC, and in a number of oxides that are candidates for “single ion ferromagnetism”, in particular SrTiO$_3$ and LiNbO$_3$.\\\\- The topic of $\\textit{p}$-type doping of nitride semiconductors shall be addressed by studying the lattice sites of the acceptor dopants Mg and Be in GaN and AlN using the short-lived probes $^{27}$Mg (9.5 min) and $^{11}$Be (13.8 s). The aim is to reach a lattice location precision around 0.05 Å in order to provide critical tests for recent theoretical models which e.g. have predicted displacements of the Mg atom from the ideal substitutional Ga and Al sites of the order...

  9. Applications of short-lived activation products in neutron activation analysis of bio-environmental specimens

    International Nuclear Information System (INIS)

    1987-03-01

    This report discusses the advantages and disadvantages, special techniques, and actual and potential applications of neutron activation analysis (NAA) utilizing short-lived neutron-induced products, with special reference to the analysis of samples of biological and environmental origin. Attention is devoted mainly to products having half-lives in roughly the range of 10 milliseconds to 60 seconds, but with some discussion of the usefulness of even shorter-lived species, and ones with half-lives as long as a few minutes. Important aspects of the analytical methodology include sample preparation, irradiation/transfer systems, activity measurements, data processing and analytical quality assurance. It is concluded that several trace elements can be determined in bio-environmental samples (as well as in samples of industrial, geochemical and other origin). In particular, this method provides analytical possibilities for several elements (e.g. B, F, Li and V) that are difficult to determine in some matrices at trace levels by any other technique. These conclusions are illustrated in an annex by results of calculations in which the applicability of the techniques to the analysis of several biological and environmental reference materials is evaluated by means of an advance computer prediction program. The report concludes with an annotated bibliography of relevant publications (including abstracts, where available) taken from the INIS database. (author)

  10. High rate gamma spectroscopy system for activation analysis of short-lived isomeric transitions

    Energy Technology Data Exchange (ETDEWEB)

    Westphall, G P [Atominstitut der Oesterreichischen Hochschulen, Vienna

    1976-07-15

    A high rate spectroscopy system specially suited for measurement of short-lived isomeric transitions is described, which, as part of a fast activation analysis facility at the TRIGA Mark II reactor, provides for automatic recording and immediate evaluation of gamma spectra taken from nuclides activated at stationary or pulsed reactor power. The system consists of a commercial de-coupled Ge(Li)-detector of 70 cm/sup 3/ modified for recycling operation for input rates in excess of 500000 c/s /sup 60/Co, a time variant trapezoidal shaping section and a fast constant dead-time ADC coupled to a programmed multichannel analyzer. Novel circuits for efficient pile-up rejection and time variant base line restoration extend the concept of gated integration up to count rates of more than 200000 c/s /sup 60/Co. Time-sequenced recording of spectra is performed by a minicomputer operated as a front-end processor of a larger laboratory computer, where final data processing takes place. New concepts for very simple and cost-effective implementation of multichannel analyzers by means of general purpose small computers are described.

  11. Dissolved organic matter composition drives the marine production of brominated very short-lived substances.

    Science.gov (United States)

    Liu, Yina; Thornton, Daniel C O; Bianchi, Thomas S; Arnold, William A; Shields, Michael R; Chen, Jie; Yvon-Lewis, Shari A

    2015-03-17

    Brominated very short-lived substances (BrVSLS), such as bromoform, are important trace gases for stratospheric ozone chemistry. These naturally derived trace gases are formed via bromoperoxidase-mediated halogenation of dissolved organic matter (DOM) in seawater. Information on DOM type in relation to the observed BrVSLS concentrations in seawater, however, is scarce. We examined the sensitivity of BrVSLS production in relation to the presence of specific DOM moieties. A total of 28 model DOM compounds in artificial seawater were treated with vanadium bromoperoxidase (V-BrPO). Our results show a clear dependence of BrVSLS production on DOM type. In general, molecules that comprise a large fraction of the bulk DOM pool did not noticeably affect BrVSLS production. Only specific cell metabolites and humic acid appeared to significantly enhance BrVSLS production. Amino acids and lignin phenols suppressed enzyme-mediated BrVSLS production and may instead have formed halogenated nonvolatile molecules. Dibromomethane production was not observed in any experiments, suggesting it is not produced by the same pathway as the other BrVSLS. Our results suggest that regional differences in DOM composition may explain the observed BrVSLS concentration variability in the global ocean. Ultimately, BrVSLS production and concentrations are likely affected by DOM composition, reactivity, and cycling in the ocean.

  12. Short-Lived Electronically-Excited Diatomic Molecules Cooled via Supersonic Expansion from a Plasma Microjet

    Science.gov (United States)

    Houlahan, Thomas J., Jr.; Su, Rui; Eden, Gary

    2014-06-01

    Using a pulsed plasma microjet to generate short-lived, electronically-excited diatomic molecules, and subsequently ejecting them into vacuum to cool via supersonic expansion, we are able to monitor the cooling of molecules having radiative lifetimes as low as 16 ns. Specifically, we report on the rotational cooling of He_2 molecules in the d^3Σ_u^+, e^3Π_g, and f^3Σ_u^+ states, which have lifetimes of 25 ns, 67 ns, and 16 ns, respectively. The plasma microjet is driven with a 2.6 kV, 140 ns high-voltage pulse (risetime of 20 ns) which, when combined with a high-speed optical imaging system, allows the nonequilibrium rotational distribution for these molecular states to be monitored as they cool from 1200 K to below 250 K with spatial and temporal resolutions of below 10 μm and 10 ns, respectively. The spatial and temporal resolution afforded by this system also allows the observation of excitation transfer between the f^3Σ_u^+ state and the lower lying d^3Σ_u^+ and e^3Π_g states. The extension of this method to other electronically excited diatomics with excitation energies >5 eV will also be discussed.

  13. Sizes and shapes of short-lived nuclei via laser spectroscopy. Final report

    International Nuclear Information System (INIS)

    Lewis, D.A.

    1985-10-01

    This project, a collaboration involving Iowa State University, Argonne National Lab., and the University of Minnesota, was aimed at the determination of properties of short-lived nuclei through their atomic hyperfine structure and optical isotope shifts. The basic approach was to use a cryogenic He-jet system to thermalize, neutralize, and transport radioactive nuclei produced online into a region suitable for laser spectroscopy. The photon burst method was then used for high sensitivity with the resulting continuous atomic beam. The experiment was located on beamline of the ANL superconducting heavy-ion accelerator. The He-jet system developed would reliably transport approx.10 2 nuclei into phase space useful for high resolution laser spectroscopy. The laser system developed could accurately and reproducibly sweep small frequency ranges for periods greater than or equal to1 day and sensitivity limits less than or equal to1 atom/s were achieved. However the nuclei were not transported as free atoms precluding nuclear determinations. Attempts to obtain free atoms by eliminating turbulence and contamination were not successful. Some of the high sensitivity spectroscopy techniques developed in this work are now being applied in a search for nuclear relics of the Big Bang and in studies of the photon statistics of light scattered by a single atom. 3 refs., 4 figs

  14. Impact on short-lived climate forcers increases projected warming due to deforestation.

    Science.gov (United States)

    Scott, C E; Monks, S A; Spracklen, D V; Arnold, S R; Forster, P M; Rap, A; Äijälä, M; Artaxo, P; Carslaw, K S; Chipperfield, M P; Ehn, M; Gilardoni, S; Heikkinen, L; Kulmala, M; Petäjä, T; Reddington, C L S; Rizzo, L V; Swietlicki, E; Vignati, E; Wilson, C

    2018-01-11

    The climate impact of deforestation depends on the relative strength of several biogeochemical and biogeophysical effects. In addition to affecting the exchange of carbon dioxide (CO 2 ) and moisture with the atmosphere and surface albedo, vegetation emits biogenic volatile organic compounds (BVOCs) that alter the formation of short-lived climate forcers (SLCFs), which include aerosol, ozone and methane. Here we show that a scenario of complete global deforestation results in a net positive radiative forcing (RF; 0.12 W m -2 ) from SLCFs, with the negative RF from decreases in ozone and methane concentrations partially offsetting the positive aerosol RF. Combining RFs due to CO 2 , surface albedo and SLCFs suggests that global deforestation could cause 0.8 K warming after 100 years, with SLCFs contributing 8% of the effect. However, deforestation as projected by the RCP8.5 scenario leads to zero net RF from SLCF, primarily due to nonlinearities in the aerosol indirect effect.

  15. Context of the long-term management of low-level short-lived waste

    International Nuclear Information System (INIS)

    Hooft, E.

    2004-01-01

    Until the international moratorium of 1983, Belgium relied on sea disposal for its low-level waste. Since then, ONDRAF/NIRAS, the Belgian radioactive waste management agency, has launched studies to look for land-based solutions. These studies, which are still going on, have gone through various phases. The sometimes harsh reactions in public opinion and the recommendations of independent experts, however, progressively led ONDRAF/NIRAS to question its work methodology. On 16 January 1998 was a milestone in Belgian's nuclear waste management. On that day, the Belgian federal government opted for a final, or potentially final, solution for the long-term management of short-lived, low-level radioactive waste, a solution that also had to be progressive, flexible, and reversible. At the same time, the government entrusted new missions to ONDRAF/NIRAS in particular that of developing methods to enable the integration of final repository project proposals at a local level and restricted the number of potential sites for final disposal to the four existing nuclear sites in Belgium and to possibly interested local districts. The government's decision of 16 January 1998 forced ONDRAF/NIRAS to change its strategy. The agency set up a new work programme and worked out an innovative methodology. This new methodology aims to generate, at the level of the interested towns and villages, draft projects for a final repository supported by a wide public consensus. (author)

  16. A high rate gamma spectroscopy system for activation analysis of short lived isomeric transitions

    Energy Technology Data Exchange (ETDEWEB)

    Westphal, G P [Atominstitut, Vienna (Austria)

    1976-07-01

    A high rate spectroscopy system specially suited for measurement of short-lived isomeric transitions is described, which, as part of a fast activation analysis facility at the TRIGA Mark II reactor, provides for automatic recording and immediate evaluation of gamma spectra taken from nuclides activated at stationary or pulsed reactor power. The system consists of a commercial DC-coupled Ge(Li)-detector of 70 cm{sup 3} modified for recycling operation for input rates in excess of 500,000 c/s Co-60, a time variant trapezoidal shaping section and a fast constant dead-time ADC coupled to a programmed multi-channel analyzer. Novel circuits for efficient pile-up rejection and time variant base line restoration extend the concept of gated integration up to count rates of more than 300,000 c/s Co-60. Time-sequenced recording of spectra is performed by a mini computer operated as a front-end processor of a larger laboratory computer, where final data processing takes place. New concepts for very simple and cost-effective implementation of multi-channel analyzers by means of general purpose small computers are described. (author)

  17. Radionuclide trap

    International Nuclear Information System (INIS)

    McGuire, J.C.

    1978-01-01

    The deposition of radionuclides manganese-54, cobalt-58 and cobalt-60 from liquid sodium coolant is controlled by providing surfaces of nickel or high nickel alloys to extract the radionuclides from the liquid sodium, and by providing surfaces of tungsten, molybdenum or tantalum to prevent or retard radionuclide deposition

  18. Radioactive fallout and neural tube defects

    Directory of Open Access Journals (Sweden)

    Nejat Akar

    2015-10-01

    Full Text Available Possible link between radioactivity and the occurrence of neural tube defects is a long lasting debate since the Chernobyl nuclear fallout in 1986. A recent report on the incidence of neural defects in the west coast of USA, following Fukushima disaster, brought another evidence for effect of radioactive fallout on the occurrence of NTD’s. Here a literature review was performed focusing on this special subject.

  19. Radioactivity monitoring of fallout, water and ground

    International Nuclear Information System (INIS)

    Radosavljevic, R.

    1961-01-01

    During 1961, the radioactivity monitoring of the Boris Kidric Institute site covered monitoring of the total β activity of the fallout and water on the site. Activity of the fallout was monitored by measuring the activity of the rain and collected sedimented dust form the atmosphere. Water monitored was the water from Danube and river Mlaka, technical and drinking water. Plants and soil activity were not measured although sample were taken and the total β activity will be measured and analysed later

  20. Vegetation fires, smoke emissions, and dispersion of radionuclides in the chernobyl exclusion zone

    Science.gov (United States)

    Wei Min Hao; Oleg O. Bondarenko; Sergiy Zibtsev; Diane Hutton

    2009-01-01

    The accident of the Chernobyl nuclear power plant (ChNPP) in 1986 was probably the worst environmental disaster in the past 30 years. The fallout and accumulation of radionuclides in the soil and vegetation could have long-term impacts on the environment. Radionuclides released during large, catastrophic vegetation fires could spread to continental Europe, Scandinavia...

  1. Radioactive fallout from Chinese nuclear weapons test of March 15, 1978

    International Nuclear Information System (INIS)

    Thomas, C.W.

    1979-01-01

    Pacific Northwest Laboratory (PNL) has measured the radionuclide concentration of short-lived debris from a radioactive cloud, produced by a nuclear weapons test conducted by the People's Republic of China on March 15, 1978. Analysis with a 40 cfm Sierra impactor showed that a large portion of the radioactivity was associated with relatively large particles. Surface air samples showed significant concentrations of 124 Sb. Samples of rain water from New York State showed that radioactivity arrived on the east coast at about the same time as peak debris levels were observed on the west coast. Highest concentrations of 131 I occurred along the Washington State--Canadian border

  2. Determination of gamma-ray exposure rate from short-lived fission products under criticality accident conditions

    International Nuclear Information System (INIS)

    Yanagisawa, Hiroshi; Ohno, Akio; Aizawa, Eijyu

    2002-01-01

    For the assessment of γ-ray doses from short-lived fission products (FPs) under criticality accident conditions, γ-ray exposure rates varying with time were experimentally determined in the Transient Experiment Critical Facility (TRACY). The data were obtained by reactivity insertion in the range of 1.50 to 2.93$. It was clarified from the experiments that the contribution of γ-ray from short-lived FPs to total exposure during the experiments was evaluated to be 15 to 17%. Hence, the contribution cannot be neglected for the assessment of γ-ray doses under criticality accident conditions. Computational analyses also indicated that γ-ray exposure rates from short-lived FPs calculated with the Monte Carlo code, MCNP4B, and photon sources based on the latest FP decay data, the JENDL FP Decay Data File 2000, well agreed with the experimental results. The exposure rates were, however, extremely underestimated when the photon sources were obtained by the ORIGEN2 code. The underestimation is due to lack of energy-dependent photon emission data for major short-lived FP nuclides in the photon database attached to the ORIGEN2 code. It was also confirmed that the underestimation arose in 1,000 or less of time lapse after an initial power burst. (author)

  3. Sizes and shapes of short-lived nuclei via laser spectroscopy. Progress report, May 1, 1980-January 31, 1981

    International Nuclear Information System (INIS)

    Lewis, D.A.

    1981-02-01

    The first stage of the program to study the sizes and shapes of short-lived nuclei through their atomic hyperfine structure is to develop a movable laser spectroscopy system. This system is now almost complete and is described in this report along with plans for measurements at Argonne National Laboratory and Brookhaven National Laboratory

  4. Building Protection Against External Ionizing Fallout Radiation

    Energy Technology Data Exchange (ETDEWEB)

    Dillon, Michael B. [Lawrence Livermore National Lab. (LLNL), Livermore, CA (United States); Homann, Steven G. [Lawrence Livermore National Lab. (LLNL), Livermore, CA (United States)

    2016-12-01

    A nuclear explosion has the potential to injure or kill tens to hundreds of thousands of people through exposure to fallout (external gamma) radiation. Existing buildings can protect their occupants (reducing external radiation exposures) by placing material and distance between fallout particles and indoor individuals. This protection is not well captured in current fallout risk assessment models and so the US Department of Defense is implementing the Regional Shelter Analysis methodology to improve the ability of the Hazard Prediction and Assessment Capability (HPAC) model to account for building protection. This report supports the HPAC improvement effort by identifying a set of building attributes (next page) that, when collectively specified, are sufficient to calculate reasonably accurate, i.e., within a factor of 2, fallout shelter quality estimates for many individual buildings. The set of building attributes were determined by first identifying the key physics controlling building protection from fallout radiation and then assessing which building attributes are relevant to the identified physics. This approach was evaluated by developing a screening model (PFscreen) based on the identified physics and comparing the screening model results against the set of existing independent experimental, theoretical, and modeled building protection estimates. In the interests of transparency, we have developed a benchmark dataset containing (a) most of the relevant primary experimental data published by prior generations of fallout protection scientists as well as (b) the screening model results.

  5. Manual estimation of fallout casualties. Final report

    International Nuclear Information System (INIS)

    Gant, K.S.; Haaland, C.M.

    1978-08-01

    A method is described for enabling Emergency Operating Centers (EOCs) to estimate nuclear fallout casualties (fatalities and injuries) during and after nuclear attack without the aid of computers. This method is compatible with the current manual method for estimating initial weapons effects. The new technique requires that the EOCs have information on nuclear detonations and upper wind conditions and that they have maps, a protractor, map overlay material, grease pencils, worksheets, and pencils. In addition, they will need two tables of data and a fallout casualty (FC) template, all supplied in this report. Five steps are involved in the estimation of fallout casualties for an area: sketching fallout wind streamlines on a map overlay; plotting locations of nuclear detonations and their fallout streamlines; measuring crosswind and upwind distances to detonation points from the point of interest; reading radiation exposure tables and summing the contributions from different weapons to obtain the exposure at that point; and using the FC template with the protection factor profile for the area to estimate fatalities and injuries. The tables of radiation exposure are based on a modified Weapons Systems Evaluation Group-10 (WSEG-10) fallout model. The table of county protection factor profiles (PFPs) assumes a Community Shelter Plan (CSP) posture

  6. Design and Performance Assessment of a Conceptual Cover Cap of Near Surface Repository for Short Lived Low and Intermediate Level Radioactive Waste

    Energy Technology Data Exchange (ETDEWEB)

    Asaba, Ruth; Kim, Changlak [KEPCO International Nuclear Graduate School, Ulsan (Korea, Republic of)

    2014-05-15

    The safety of the overall waste disposal system is determined by the performance of its individual components: waste form, waste container, engineered barrier and the host environment. The design of the cover cap helps in preventing percolation of water, and in retarding radionuclide migration from the disposal facility to the biosphere. The cover of a disposal facility is usually a combination of materials such as sand, gravel, concrete, clay and soil conditioned for vegetation growth. The cover system will be designed using models such as EPA's Hydrological Evaluation of Land fill Performance (HELP) code. This paper describes a conceptual design for a cover cap for a land fill as a preferred disposal facility for low and short lived intermediate radioactive waste in Uganda. Majority of the waste is generated from disused sealed and unsealed radioactive sources arising from medical, industrial applications, and research. Radioactive waste management has raised a lot of concern in both developed and developing countries. Each country has a responsibility to come up with a solution to prevent contamination of the environment and humans from radioactive waste. It is important to have thicker soil layers in cap designs so as to support vegetation growth since some activities such as erosion and settlements are expected. Help simulations in this study will assist to demonstrate that it is possible to design a cover cap which can contain radioactive waste packages for hundreds of years provided the proper institutional and performance monitoring schemes are implemented.

  7. A proposal for assessing study quality: Biomonitoring, Environmental Epidemiology, and Short-lived Chemicals (BEES-C) instrument

    Science.gov (United States)

    LaKind, Judy S.; Sobus, Jon R.; Goodman, Michael; Barr, Dana Boyd; Fürst, Peter; Albertini, Richard J.; Arbuckle, Tye E.; Schoeters, Greet; Tan, Yu-Mei; Teeguarden, Justin; Tornero-Velez, Rogelio; Weisel, Clifford P.

    2015-01-01

    The quality of exposure assessment is a major determinant of the overall quality of any environmental epidemiology study. The use of biomonitoring as a tool for assessing exposure to ubiquitous chemicals with short physiologic half-lives began relatively recently. These chemicals present several challenges, including their presence in analytical laboratories and sampling equipment, difficulty in establishing temporal order in cross-sectional studies, short- and long-term variability in exposures and biomarker concentrations, and a paucity of information on the number of measurements required for proper exposure classification. To date, the scientific community has not developed a set of systematic guidelines for designing, implementing and interpreting studies of short-lived chemicals that use biomonitoring as the exposure metric or for evaluating the quality of this type of research for WOE assessments or for peer review of grants or publications. We describe key issues that affect epidemiology studies using biomonitoring data on short-lived chemicals and propose a systematic instrument – the Biomonitoring, Environmental Epidemiology, and Short-lived Chemicals (BEES-C) instrument – for evaluating the quality of research proposals and studies that incorporate biomonitoring data on short-lived chemicals. Quality criteria for three areas considered fundamental to the evaluation of epidemiology studies that include biological measurements of short-lived chemicals are described: 1) biomarker selection and measurement, 2) study design and execution, and 3) general epidemiological study design considerations. We recognize that the development of an evaluative tool such as BEES-C is neither simple nor non-controversial. We hope and anticipate that the instrument will initiate further discussion/debate on this topic. PMID:25137624

  8. Distribution of anthropogenic and naturally occurring radionuclides in soils and lakes of Central Spitsbergen (Arctic)

    International Nuclear Information System (INIS)

    Lokas, Edyta

    2017-01-01

    This work provides the first results on activity concentrations, inventories and activity ratios of the artificial and natural fallout ("1"3"7Cs, "2"3"8Pu, "2"3"9"+"2"4"0Pu, "2"4"1Am, "2"1"0Pb) and lithogenic radionuclides ("2"2"6Ra, "2"2"8Ra, "4"0K) in soils and lake sediments of the inland Spitsbergen. The depths of activity peaks of the artificial radionuclides point to accumulation of up to 10 cm thick deposits during last 50 years. The activity ratios of the radionuclides suggest global fallout as their source. Despite low annual precipitation the inventories of fallout radionuclides in sites not affected by the secondary deposition agree with those reported from the more humid areas of Spitsbergen. (author)

  9. Convective Transport of Very-short-lived Bromocarbons to the Stratosphere

    Science.gov (United States)

    Liang, Qing; Atlas, Elliot Leonard; Blake, Donald Ray; Dorf, Marcel; Pfeilsticker, Klaus August; Schauffler, Sue Myhre

    2014-01-01

    We use the NASA GEOS Chemistry Climate Model (GEOSCCM) to quantify the contribution of two most important brominated very short-lived substances (VSLS), bromoform (CHBr3) and dibromomethane (CH2Br2), to stratospheric bromine and its sensitivity to convection strength. Model simulations suggest that the most active transport of VSLS from the marine boundary layer through the tropopause occurs over the tropical Indian Ocean, the Western Pacific warm pool, and off the Pacific coast of Mexico. Together, convective lofting of CHBr3 and CH2Br2 and their degradation products supplies 8 ppt total bromine to the base of the Tropical Tropopause Layer (TTL, 150 hPa), similar to the amount of VSLS organic bromine available in the marine boundary layer (7.8-8.4 ppt) in the above active convective lofting regions. Of the total 8 ppt VSLS-originated bromine that enters the base of TTL at 150 hPa, half is in the form of source gas injection (SGI) and half as product gas injection (PGI). Only a small portion (Br2, together, contribute 7.7 pptv to the present-day inorganic bromine in the stratosphere. However, varying model deep convection strength between maximum and minimum convection conditions can introduce a 2.6 pptv uncertainty in the contribution of VSLS to inorganic bromine in the stratosphere (BryVSLS). Contrary to the conventional wisdom, minimum convection condition leads to a larger BryVSLS as the reduced scavenging in soluble product gases, thus a significant increase in PGI (2-3 ppt), greatly exceeds the relative minor decrease in SGI (a few 10ths ppt.

  10. A growing threat to the ozone layer from short-lived anthropogenic chlorocarbons

    Directory of Open Access Journals (Sweden)

    D. E. Oram

    2017-10-01

    Full Text Available Large and effective reductions in emissions of long-lived ozone-depleting substance (ODS are being achieved through the Montreal Protocol, the effectiveness of which can be seen in the declining atmospheric abundances of many ODSs. An important remaining uncertainty concerns the role of very short-lived substances (VSLSs which, owing to their relatively short atmospheric lifetimes (less than 6 months, are not regulated under the Montreal Protocol. Recent studies have found an unexplained increase in the global tropospheric abundance of one VSLS, dichloromethane (CH2Cl2, which has increased by around 60 % over the past decade. Here we report dramatic enhancements of several chlorine-containing VSLSs (Cl-VSLSs, including CH2Cl2 and CH2ClCH2Cl (1,2-dichloroethane, observed in surface and upper-tropospheric air in East and South East Asia. Surface observations were, on occasion, an order of magnitude higher than previously reported in the marine boundary layer, whilst upper-tropospheric data were up to 3 times higher than expected. In addition, we provide further evidence of an atmospheric transport mechanism whereby substantial amounts of industrial pollution from East Asia, including these chlorinated VSLSs, can rapidly, and regularly, be transported to tropical regions of the western Pacific and subsequently uplifted to the tropical upper troposphere. This latter region is a major provider of air entering the stratosphere, and so this mechanism, in conjunction with increasing emissions of Cl-VSLSs from East Asia, could potentially slow the expected recovery of stratospheric ozone.

  11. Regional scale temperature and circulation impacts of short-lived climate pollutants reductions

    Science.gov (United States)

    Oudar, T.; Kushner, P. J.; Fyfe, J. C.; von Salzen, K.; Shrestha, R.

    2017-12-01

    The role of anthropogenic aerosols on climate is still not clearly understood. Aerosol forcing is spatially heterogeneous and their emissions are controlled by regional economic and regulatory factors. For example, it is known that black carbon is responsible for a global net warming but its regional impacts are less understood. We evaluate the regional climate impacts of anthropogenic aerosol emission changes over the recent past and near future. Specifically, we report on numerical experiments using aerosol emissions from the Evaluating the Climate and Air Quality Impacts of Short-Lived Pollutants (ECLIPSE, Stohl et al., 2015) project. These scenarios are alternative mitigation pathways for black carbon and organic aerosol over the period from 1990 to 2050. With these scenarios, we carried out three sets of simulation using the second generation Canadian Earth System Model (CanESM2): 1) A current legislation emission (CLE) scenario for black carbon and organic aerosols; 2) A mitigation (MIT) scenario for black carbon and organic aerosols, and; 3) A black carbon only mitigation scenario (MIT-BC). Five simulations were carried out for each scenario and the response analyzed in the context of a large fifty-member initial condition ensemble of simulations using historical anthropogenic aerosol forcings to 2005 as well as those forcing from the RCP8.5 scenario to 2020. Our main finding is a significant springtime cooling over the Northern midlatitudes that attributable to black carbon. Other cooling signals attributable to black carbon reductions are found in the boreal summer over Southern Europe as well as over the Northern Hemisphere midlatitudes and tropical troposphere in boreal summer and fall. All of these cooling signals are to some degree offset by simultaneous reductions in organic aerosols. As a check on the robustness, we will also report on results of five-member draws from the large ensemble over periods of comparably strong radiative forcing changes, to

  12. Extreme radionuclide accumulation on alpine glaciers in cryoconites

    International Nuclear Information System (INIS)

    Lettner, H.; Wilflinger, T.; Hubmer, A.K.; Bossew, P.

    2008-01-01

    Full text: Under environmental conditions when radionuclide fallout will not be diluted by media like soil or water, radionuclides deposited may accumulate to unusual high activities. On glacier surfaces conditions as such exist for aerosols and airborne dust deposited with anthropogenic and natural radionuclides attached on their surfaces. In the course of agglomeration processes initiated by melting and redistribution, these particles may concentrate in small depressions, ice pockets, ablation edges etc. and form substances called cryoconites ('ice dust'). As there is no other matrix than the original aerosol particles, cryoconites are a sink for radionuclides and airborne pollutants and their activity levels are among the highest produced by natural processes observed in environmental media. 137 Cs activities found on glaciers in the Austrian alps are between 255 and 136.000 Bq/kg and predominantly derived from Chernobyl, but also from global fallout. Further anthropogenic radionuclides detected are 134 Cs, 90 Sr, 238,239+240 Pu, 241 Am, 125 Sb, 154 Eu, 60 Co and 207 Bi. In combination with the naturally occurring radionuclides 7 Be and 210 Pb and isotopic ratios such as 134 Cs/ 137 Cs, identification and discrimination of the sources, the nuclear weapon tests and the Chernobyl fallout, can be carried out. (author)

  13. Peculiarities of radionuclide transfer to plants

    International Nuclear Information System (INIS)

    Butkus, D.; Andriulaityte, I.; Luksiene, B.; Druteikiene, R.

    2003-01-01

    The biosphere and its interacting components (air, soil, bottom sediments, flora, fauna, human beings) are constantly affected by ionizing radiation. One of the ionizing radiation sources is noble radioactive gas that is continually released into the environment because of the normal operation of nuclear power plants (short-lived and long-lived noble gas) and nuclear fuel-reprocessing plants (long-lived noble gas). Another source is related to nuclear tests and the Chernobyl NPP accident, when long-lived gaseous and aerosol radionuclides ( 85 Kr, transuranics, 137 Cs, 90 Sr, etc) were spread in all environmental systems. In order to evaluate the mechanism of radionuclide transfer to plants, model experimental investigation using gaseous 85 Kr and ionic state 137 Cs was undertaken. For this purpose specific chambers with defined physical parameters were applied. The gained tentative results show the importance of these experiments for the estimation of radionuclide transfer to plants and for the prognosis of human internal irradiation. (author)

  14. Late radiation effects in Marshall Islanders exposed to fallout 28 years ago

    International Nuclear Information System (INIS)

    Conard, R.A.

    1984-01-01

    In 1954, following detonation of a megaton nuclear device at Bikini, an unfortunate accident occurred owing to an unpredicted shift in winds resulting in exposure to radioactive fallout of 250 Marshallese people, 28 American servicemen on atolls to the east, and 23 Japanese fishermen on their fishing vessel. In this presentation, medical findings in the exposed Marshallese noted over the past 28 years is briefly reviewed with particular emphasis on late effects on the thyroid gland. The Marshallese were too far distant from the detonation for any direct effects, and their exposure was due entirely to fallout radiation during the 2 days prior to evacuation. This consisted of penetrating whole-body gamma radiation, irradiation of the skin (principally beta radiation) from fallout deposited on the skin, and internal absorption of radionuclides from ingestion of contaminated food and water. The most serious internal exposure was that to the thyroid from radioiodines, which were relatively abundant in the fallout. 63 references, 1 figure, 4 tables

  15. Mapping of caesium fallout from the Chernobyl accident in the Jotunheimen area

    International Nuclear Information System (INIS)

    Baranwal, Vikas C.; Ofstad, Frode; Roenning, Jan S.; Watson, Robin J.

    2011-01-01

    As a consequence of the Chernobyl accident, several areas in Norway received radioactive fallout. One of these areas is the eastern part of Jotunheimen in central Norway. Immediately after the accident in 1986, the Geological Survey of Norway (NGU) performed airborne gamma-ray spectroscopy in central Norway. At that time, it was not possible to calculate reliable radionuclide concentrations, and the data were presented as total counts per second. Several man-made radionuclides were present in the initial fallout, but due to short half-lives, most of these have now disintegrated into stable isotopes. 137Cs, with a half-life of 11.000 days (∼ 30 years) is still present in the environment in significant quantities, leading to high radioactivity levels in meat from reindeer and sheep. To obtain a detailed map of the caesium fallout concentration in Jotunheimen, an airborne gamma-ray spectrometry (AGRS) survey was carried out, focusing on reindeer grazing areas. This project was a cooperation between Reindeer Husbandry Administration, Norwegian Radiation Protection Authority and the Geological Survey of Norway.(Au)

  16. Mapping of caesium fallout from the Chernobyl accident in the Jotunheimen area

    Energy Technology Data Exchange (ETDEWEB)

    Baranwal, Vikas C.; Ofstad, Frode; Roenning, Jan S.; Watson, Robin J.

    2011-07-01

    As a consequence of the Chernobyl accident, several areas in Norway received radioactive fallout. One of these areas is the eastern part of Jotunheimen in central Norway. Immediately after the accident in 1986, the Geological Survey of Norway (NGU) performed airborne gamma-ray spectroscopy in central Norway. At that time, it was not possible to calculate reliable radionuclide concentrations, and the data were presented as total counts per second. Several man-made radionuclides were present in the initial fallout, but due to short half-lives, most of these have now disintegrated into stable isotopes. 137Cs, with a half-life of 11.000 days ({approx} 30 years) is still present in the environment in significant quantities, leading to high radioactivity levels in meat from reindeer and sheep. To obtain a detailed map of the caesium fallout concentration in Jotunheimen, an airborne gamma-ray spectrometry (AGRS) survey was carried out, focussing on reindeer grazing areas. This project was a cooperation between Reindeer Husbandry Administration, Norwegian Radiation Protection Authority and the Geological Survey of Norway. (auth)

  17. Measurements of atmospheric fallout in Argentina; Determinacion del fallout atmosferico en la Republica Argentina

    Energy Technology Data Exchange (ETDEWEB)

    Canoba, A C; Lopez, F O; Bruno, H A

    1998-11-01

    With the purpose of studying the radioactive fallout present in Argentina from atmospheric nuclear explosions tests that have been conducted recently, an environmental monitoring program, outside the influence of nuclear facilities of Argentina, was undertaken during 1996 and 1997. The levels of Cs-137 and Sr-90 were analysed in samples of air, deposited material (rainwater), milk, an average meal of a standard man and food. During this period, a total of 630 radiochemical analysis were performed on 325 samples of the different matrices described. The concentration levels of the radionuclides analysed in the different environmental matrices are presented and are compared with the values obtained in the environmental monitoring program done during the period 1960-1981. (author) 3 refs., 9 tabs. [Espanol] Con el proposito de estudiar la precipitacion radiactiva presente en la Republica Argentina, debido al ensayo de armas nucleares en la atmosfera realizadas en el pasado, se implemento el muestreo ambiental fuera de la zona de influencia de las instalaciones nucleares de la Argentina durante los anios 1996 y 1997. Se determinaron las concentraciones de cesio 137 y estroncio 90 en muestras de aire, deposito de material radiactivo (agua de lluvia), leche, dieta promedio de un individuo estandar y en alimentos varios. Se realizaron, durante el periodo mencionado, un total de 630 determinaciones radioquimicas sobre 325 muestras de las diferentes matrices mencionadas. Se presentan los niveles de concentracion de los radionucleidos analizados en las distintas matrices ambientales y se comparan los valores obtenidos en los monitoreos realizados durante el periodo 1960-1981. (autor)

  18. Radionuclide toxicity

    International Nuclear Information System (INIS)

    Galle, P.

    1982-01-01

    The aim of this symposium was to review the radionuclide toxicity problems. Five topics were discussed: (1) natural and artificial radionuclides (origin, presence or emission in the environment, human irradiation); (2) environmental behaviour of radionuclides and transfer to man; (3) metabolism and toxicity of radionuclides (radioiodine, strontium, rare gas released from nuclear power plants, ruthenium-activation metals, rare earths, tritium, carbon 14, plutonium, americium, curium and einsteinium, neptunium, californium, uranium) cancerogenous effects of radon 222 and of its danghter products; (4) comparison of the hazards of various types of energy; (5) human epidemiology of radionuclide toxicity (bone cancer induction by radium, lung cancer induction by radon daughter products, liver cancer and leukaemia following the use of Thorotrast, thyroid cancer; other site of cancer induction by radionuclides) [fr

  19. Dormancy and germination in short-lived lepidium perfoliatu l. (brassicaceae) seeds

    International Nuclear Information System (INIS)

    Tang, An-Jun; Tian, M.; Long, Chun-Lin

    2010-01-01

    To understand germination timing in an ecological context, the response to environmental events that effect seed dormancy is central and has to be combined with knowledge of germination responses to different ecological factors. In this study, seed dormancy, germination and seedling survival of annual short-lived clasping pepper weed Lepidium perfoliatum L. (Brassicaceae) were investigated. Three types of pre-treatments viz., various temperature dry storage, light and water stress were tested as possible dormancy and survival-affecting environmental events. Fresh mature seeds were greatly dormant. Warm (30 deg. C) dry storage more facilitated breaking dormancy, they germinated well under apt conditions (e.g. 20 deg. C and 10/20 deg. C plus periodic light, 14 h/d). For those seeds which underwent after-ripening, they could germinate at a range of constant temperatures (4, 10, 15, 20, 25, and 30 deg. C) and one alternating temperature (10/20 deg. C). Under alternating temperature regimes, the final percent germination of L. perfoliatum seeds increased from 37 deg. C to 93% when temperature altered from 4/10 deg. C to 10/20 deg. C in light, then decreased with increasing temperature. The germination pattern under constant temperature conditions was similar to that under alternating temperature and significant differences in final percent germinations and rates of germination were observed among different temperatures. Under different light treatments, final germination of showed significant differences, only with 35% of germination percentage in dark, much lower than those in red and white light (i.e. 93% and 91%, respectively). GA3 could promote the germination of non-dormant seeds in dark. When water potentials were reduced, final percent germination decreased dramatically, and few seeds germinated at -0.98 MPa (generated by PEG-8000). The changes of proline content in resultant seedlings were reverse to that of final percent germination with changing water

  20. Seasonal variation in the behaviour of a short-lived rodent.

    Science.gov (United States)

    Eccard, Jana A; Herde, Antje

    2013-11-15

    Short lived, iteroparous animals in seasonal environments experience variable social and environmental conditions over their lifetime. Animals can be divided into those with a "young-of-the-year" life history (YY, reproducing and dying in the summer of birth) and an "overwinter" life history (OW, overwintering in a subadult state before reproducing next spring).We investigated how behavioural patterns across the population were affected by season and sex, and whether variation in behaviour reflects the variation in life history patterns of each season. Applications of pace-of-life (POL) theory would suggest that long-lived OW animals are shyer in order to increase survival, and YY are bolder in order to increase reproduction. Therefore, we expected that in winter and spring samples, when only OW can be sampled, the animals should be shyer than in summer and autumn, when both OW and YY animals can be sampled.We studied common vole (Microtus arvalis) populations, which express typical, intra-annual density fluctuation. We captured a total of 492 voles at different months over 3 years and examined boldness and activity level with two standardised behavioural experiments. Behavioural variables of the two tests were correlated with each other. Boldness, measured as short latencies in both tests, was extremely high in spring compared to other seasons. Activity level was highest in spring and summer, and higher in males than in females. Being bold in laboratory tests may translate into higher risk-taking in nature by being more mobile while seeking out partners or valuable territories. Possible explanations include asset-protection, with OW animals being rather old with low residual reproductive value in spring. Therefore, OW may take higher risks during this season. Offspring born in spring encounter a lower population density and may have higher reproductive value than offspring of later cohorts. A constant connection between life history and animal personality, as

  1. Regional emission metrics for short-lived climate forcers from multiple models

    Directory of Open Access Journals (Sweden)

    B. Aamaas

    2016-06-01

    Full Text Available For short-lived climate forcers (SLCFs, the impact of emissions depends on where and when the emissions take place. Comprehensive new calculations of various emission metrics for SLCFs are presented based on radiative forcing (RF values calculated in four different (chemical-transport or coupled chemistry–climate models. We distinguish between emissions during summer (May–October and winter (November–April for emissions in Europe and East Asia, as well as from the global shipping sector and global emissions. The species included in this study are aerosols and aerosol precursors (BC, OC, SO2, NH3, as well as ozone precursors (NOx, CO, VOCs, which also influence aerosols to a lesser degree. Emission metrics for global climate responses of these emissions, as well as for CH4, have been calculated using global warming potential (GWP and global temperature change potential (GTP, based on dedicated RF simulations by four global models. The emission metrics include indirect cloud effects of aerosols and the semi-direct forcing for BC. In addition to the standard emission metrics for pulse and sustained emissions, we have also calculated a new emission metric designed for an emission profile consisting of a ramping period of 15 years followed by sustained emissions, which is more appropriate for a gradual implementation of mitigation policies.For the aerosols, the emission metric values are larger in magnitude for emissions in Europe than East Asia and for summer than winter. A variation is also observed for the ozone precursors, with largest values for emissions in East Asia and winter for CO and in Europe and summer for VOCs. In general, the variations between the emission metrics derived from different models are larger than the variations between regions and seasons, but the regional and seasonal variations for the best estimate also hold for most of the models individually. Further, the estimated climate impact of an illustrative mitigation

  2. Radon and its short-lived daughter products in the lower atmosphere

    International Nuclear Information System (INIS)

    Servant, J.

    1964-01-01

    The variations of vertical and temporal distributions of natural radioactivity with geographical location in the lower atmospheric layers are shown. The content of radon and its short lived daughters products are measured. Radon content is measured continually with a new apparatus, the sensibility of which is 0,2.10 -11 Ci m -3 i.e. the fiftieth of the mean concentration near the soil, this apparatus allowed us to show that radioactive equilibrium between radon and its daughter products is realised when the atmosphere is stable. Air observations between 0 and 100 meters above the ground point out that radon and its decay products are valuable tracers to mark the stability of the atmosphere. Under very stable nighttime conditions the radon accumulates in the former 30 meters of the air layer, at sunrise it ascends and at 9 o'clock attains 100 meters high. The removal rate of the air in the lower atmosphere is computed from the movement of this radon mass, it is equal to 90 per cent for a summer day. We have show that this radon comes from the soil in which it diffuses by brownian motion the intensity of which varies with the water content of the soil, its value for June 1958 is 6,10 -17 Ci cm -2 s -1 and for January 1959 0.2,10 -17 Ci cm -2 s - 1. During the year 1958-1959 general mean of flux for the sedimentary soil studied is equal to 3. 8 ± 1.3, 10 -17 Ci cm -2 s -1 it is identical to the world wide mean computed by H. Israel. In a hilly site in the Morvan, air movements are well marked by this radioactivity. We observed from one hand downslope and up-slope breezes having, respectively, speeds of 0.2 m s -1 and 0.7 m s -1 and from the other hand by night, in the valley and with a light wind favours the stagnation of the air near the ground, a strong increase of the radioactivity which is proportional to the one of the granitic rocks of the region. The radon flux of this soil is 74,10 -17 Ci cm -2 s -1 and the radioactivity of the air can attain 1.5,10 -8 Ci m

  3. The effects of fallout from nuclear explosions

    International Nuclear Information System (INIS)

    Cook, J.

    1987-01-01

    Early fallout from surface or near surface nuclear explosions leads to radiation doses at levels sufficient to cause deaths from the acute effects of radiation over large areas, particularly if no means of avoiding exposure are available. For example, early fallout from a 10 megatonne weapon could lead to doses in excess of 4 or 5 grays (at which half of those exposed die) over an area of about 25,000 square kilometres, in a deposit perhaps 400 km long and 80 km wide. The survivors of early fallout are likely to experience a significant increase in thyroid disease (for children at the time of exposure), in leukaemia and a probably detectable increase in cancer. It is unlikely that there would be any significant increase in the incidence of genetic disability and ill-health in the children of the survivors. Delayed fallout would be distributed fairly uniformly around the earth. The additional cancer and genetic risks from delayed fallout are small, the cancer risk being less than 1 per cent of natural incidence and the genetic risk being undetectable

  4. Comparison of experimental and calculated shielding factors for modular buildings in a radioactive fallout scenario

    DEFF Research Database (Denmark)

    Hinrichsen, Yvonne; Finck, Robert; Östlund, Karl

    2018-01-01

    building used was a standard prefabricated structure obtained from a commercial manufacturer. Four reference positions for the gamma radiation detectors were used inside the building. Theoretical dose rate calculations were performed using the Monte Carlo code MCNP6, and additional calculations were......Experimentally and theoretically determined shielding factors for a common light construction dwelling type were obtained and compared. Sources of the gamma-emitting radionuclides 60Co and 137Cs were positioned around and on top of a modular building to represent homogeneous fallout. The modular...... performed that compared the shielding factor for 137Cs and 134Cs. This work demonstrated the applicability of using MCNP6 for theoretical calculations of radioactive fallout scenarios. Furthermore, the work showed that the shielding effect for modular buildings is almost the same for 134Cs as for 137Cs....

  5. Radioactive rare earths from fallout for study of particle movement in the sea

    International Nuclear Information System (INIS)

    Sugihara, Thomas T.; Bowen, Vaughan T.

    1962-01-01

    As part of an extensive study of the distribution of long-lived radionuclides from fallout in the Atlantic Ocean, a large number of measurements of cerium-144 and promethium-147 concentration have been made. Comparison of these concentrations as they vary both horizontally and vertically, with simultaneously measured concentrations of strontium-90, indicates that the rare earths are generally depleted in surface water, by comparison with the nuclides known to be soluble. This observation, coupled with frequent observation of rare-earth enrichment at depth, leads us to postulate rapid vertical transport of rare earths by attachment to particles undergoing sedimentation. This is completely plausible in terms of the 'radiocolloid' behaviour generally observed for rare earths at sea-water pH. An attempt is made to interpret this study in the overall picture of the marine geochemistry of the trivalent cations, as well as to emphasize the unique and generally useful aspects of the fallout tracer experiment. (author) [fr

  6. Use of mosses and lichens for regional mapping of 137Cs fallout from the Chernobyl accident

    International Nuclear Information System (INIS)

    Steinnes, E.; Njaastad, O.

    1992-01-01

    The lichens Hypogymnia physodles and Cladonia stellaris and the moss Hylocomium splendens were studied for potential use af biomonitors of the regional distribution of 137 Cs fallout in Norway from the Chernobyl accident. While Hylocomium splendens and Cladonia stellaris showed reasonable mutual agreement, the activities recorded in the epiphytic species Hypogymnia physodes were not consistent with those of the other species, and depended strongly on whether sampling was carried out on conifers or birch. The geographical distribution of 137 Cs in the two former species was in satisfactory agreement with depostion figures obtained from analysis of surface soil, considering the heterogeneous depostion pattern of Chernobyl radioactivity. Both Hylocomium splendens and Cladonia stellaris appear well suited for regional mapping of 137 Cs fallout from nuclear accidents. Regional heavy metal deposition surveys employing Hylocomium splendens might be extended to include radionuclides if desirable. (au) (21 refs.)

  7. Evaluating the climate and air quality impacts of short-lived pollutants

    Science.gov (United States)

    Stohl, A.; Aamaas, B.; Amann, M.; Baker, L. H.; Bellouin, N.; Berntsen, T. K.; Boucher, O.; Cherian, R.; Collins, W.; Daskalakis, N.; Dusinska, M.; Eckhardt, S.; Fuglestvedt, J. S.; Harju, M.; Heyes, C.; Hodnebrog, Ø.; Hao, J.; Im, U.; Kanakidou, M.; Klimont, Z.; Kupiainen, K.; Law, K. S.; Lund, M. T.; Maas, R.; MacIntosh, C. R.; Myhre, G.; Myriokefalitakis, S.; Olivié, D.; Quaas, J.; Quennehen, B.; Raut, J.-C.; Rumbold, S. T.; Samset, B. H.; Schulz, M.; Seland, Ø.; Shine, K. P.; Skeie, R. B.; Wang, S.; Yttri, K. E.; Zhu, T.

    2015-09-01

    This paper presents a summary of the work done within the European Union's Seventh Framework Programme project ECLIPSE (Evaluating the Climate and Air Quality Impacts of Short-Lived Pollutants). ECLIPSE had a unique systematic concept for designing a realistic and effective mitigation scenario for short-lived climate pollutants (SLCPs; methane, aerosols and ozone, and their precursor species) and quantifying its climate and air quality impacts, and this paper presents the results in the context of this overarching strategy. The first step in ECLIPSE was to create a new emission inventory based on current legislation (CLE) for the recent past and until 2050. Substantial progress compared to previous work was made by including previously unaccounted types of sources such as flaring of gas associated with oil production, and wick lamps. These emission data were used for present-day reference simulations with four advanced Earth system models (ESMs) and six chemistry transport models (CTMs). The model simulations were compared with a variety of ground-based and satellite observational data sets from Asia, Europe and the Arctic. It was found that the models still underestimate the measured seasonality of aerosols in the Arctic but to a lesser extent than in previous studies. Problems likely related to the emissions were identified for northern Russia and India, in particular. To estimate the climate impacts of SLCPs, ECLIPSE followed two paths of research: the first path calculated radiative forcing (RF) values for a large matrix of SLCP species emissions, for different seasons and regions independently. Based on these RF calculations, the Global Temperature change Potential metric for a time horizon of 20 years (GTP20) was calculated for each SLCP emission type. This climate metric was then used in an integrated assessment model to identify all emission mitigation measures with a beneficial air quality and short-term (20-year) climate impact. These measures together

  8. Measurements of airborne short-lived radioactivity concentration in a PET facility at a national University hospital

    International Nuclear Information System (INIS)

    Saito, Tadashi

    2006-01-01

    National universities in Japan became under regulation of Industrial Safety and Health Law since 2004FY. One of the legal obligations is working environment measurements such as airborne radioactivity concentration in the rooms where employees handle unsealed radiation sources. Both in 2004FY and in 2005FY, measurements of airborne radioactivity concentration were carried out by two different agencies. The most prominent difference among them is the measurement for short-lived PET nuclides. In 2004FY, one agency measured the radioactivity with a Ge spectrometer at its own laboratory, whereas, in 2005FY, the other agency brought a NaI scintillation counter for gross gamma counting to the Hospital. It can be shown that detection limits for short-lived PET nuclides are in principle almost the same in both methods. It is also found that, in the actual case, gamma spectrometry with a Ge spectrometer is superior in judgement of detection of the radioactivity. (author)

  9. Possibilities of chemical isolation of element 106 from aqueous solutions according to the model experiments with short lived tungsten isotopes

    International Nuclear Information System (INIS)

    Szeglowski, Z.; Bruchertseifer, H.; Brudanin, V.B.

    1993-01-01

    A rapid method for continuous separation of short-lived tungsten isotopes from the lanthanides has been developed. It consists in transforming nuclear reaction products from the target by an aerosol jet to an absorber where the KCl particulates are dissolved in 0.2 M HF and percolating the product solution through three successively linked columns filled with ion exchange resins Dowex 50X8 (cationite), Dowex 1X8 (anionite) and again Dowex 50X8. 3 refs

  10. PANTHER Data from SOLVE-II Through CR-AVE: A Contrast Between Long and Short Lived Compounds.

    Science.gov (United States)

    Moore, F. L.; Dutton, G. S.; Elkins, J. W.; Hall, B. D.; Hurst, D. F.; Nance, J. D.; Thompson, T. M.

    2006-12-01

    PANTHER (PAN and other Trace Hydrohalocarbons ExpeRiment) is an airborne 6-channel gas chromatograph that measures approximately 20 important atmospheric trace gases whose changing burdens impact air quality, climate change and both stratospheric and tropospheric ozone. In this presentation we will contrast measurements of the long-lived compounds against the short-lived compounds. The long-lived compounds tend to have well-defined troposphere boundary conditions and develop spatial gradients due to stratospheric processing. These measurements have played a major role in quantifying stratospheric transport, stratosphere- troposphere exchange, and ozone loss. In contrast the short-lived species develop spatial and temporal gradients in the tropical tropopause layer (TTL), due to variations in the surface boundary layer concentrations and the coupling of this surface boundary layer to the TTL via convective processes. Deep convection acts like a "conveyor belt" between the source region in the boundary layer and the relatively stable TTL region, often bypassing the free troposphere where scavenging of these short lived species takes place. Loss rates due to reaction with OH and thermal decomposition are reduced in the cold, dry air of the TTL, resulting in longer survival times. Isolation of the TTL region from the free troposphere can last from days to over a month. Significant amounts of these short-lived compound and their byproducts can therefore be transported into the lower stratosphere (LS). Of particular interest are compounds that contain bromine, iodine, and sulfur, not only because of their intrinsic harmful effects in the atmosphere, but also because they have unique source and sink regions that can help to de- convolve transport.

  11. The ratio of long-lived to short-lived radon-222 progeny concentrations in ground-level air

    Energy Technology Data Exchange (ETDEWEB)

    Hoetzl, H.; Winkler, R. [Institut fuer Strahlenschutz, GSF-Forschungszentrum fuer Umwelt und Gesundheit, Neuherberg Oberschleissheim (Germany)

    1996-02-09

    The ratio of {sup 210}Pb air concentration to the short-lived radon ({sup 222}Rn) decay products concentration at ground level was investigated at a semi-rural location 10 km north of Munich, south Germany, for a period of 11 years (1982-1992). The average ratio from 132 monthly mean values has been found to be (7.5{+-}2.2) x 10{sup -5} (arithmetic mean{+-}S.D.). While the time series of the short-lived radon daughter concentration exhibit a distinct seasonal pattern with maxima mostly in October of each year, the course of {sup 210}Pb air concentration is characterized by high values from October through February. Consequently, high ratios of {sup 210}Pb to short-lived decay product concentration are often observed in the winter months of December-February. To study the influence of meteorological conditions on this behaviour, {sup 210}Pb and {sup 214}Pb concentrations were measured on a short-term basis with sampling intervals of 2-3 days from October 1991 to November 1992. The air concentrations obtained within those intervals were then correlated with actual meteorological parameters. On the base of this investigation the seasonal behaviour can essentially be explained by the more frequent inversion weather conditions in winter than in the summer months. At the same location, the average ratio of {sup 210}Po to {sup 210}Pb concentration in ground level air has been found to be 0.079 from 459 weakly mean values between 1976 and 1985. Hence, the corresponding average ratios of the short-lived radon daughters (EEC) to {sup 210}Pb and {sup 210}Po, were 1:7.5x10{sup -5} and 1:0.6 x 10{sup -5}, respectively.

  12. The ratio of long-lived to short-lived radon-222 progeny concentrations in ground-level air

    International Nuclear Information System (INIS)

    Hoetzl, H.; Winkler, R.

    1996-01-01

    The ratio of 210 Pb air concentration to the short-lived radon ( 222 Rn) decay products concentration at ground level was investigated at a semi-rural location 10 km north of Munich, south Germany, for a period of 11 years (1982-1992). The average ratio from 132 monthly mean values has been found to be (7.5±2.2) x 10 -5 (arithmetic mean±S.D.). While the time series of the short-lived radon daughter concentration exhibit a distinct seasonal pattern with maxima mostly in October of each year, the course of 210 Pb air concentration is characterized by high values from October through February. Consequently, high ratios of 210 Pb to short-lived decay product concentration are often observed in the winter months of December-February. To study the influence of meteorological conditions on this behaviour, 210 Pb and 214 Pb concentrations were measured on a short-term basis with sampling intervals of 2-3 days from October 1991 to November 1992. The air concentrations obtained within those intervals were then correlated with actual meteorological parameters. On the base of this investigation the seasonal behaviour can essentially be explained by the more frequent inversion weather conditions in winter than in the summer months. At the same location, the average ratio of 210 Po to 210 Pb concentration in ground level air has been found to be 0.079 from 459 weakly mean values between 1976 and 1985. Hence, the corresponding average ratios of the short-lived radon daughters (EEC) to 210 Pb and 210 Po, were 1:7.5x10 -5 and 1:0.6 x 10 -5 , respectively

  13. The "AQUASCOPE" simplified model for predicting 89, 90Sr, 131l and 134, 137Cs in surface waters after a large-scale radioactive fallout

    NARCIS (Netherlands)

    Smith, J.T.; Belova, N.V.; Bulgakov, A.A.; Comans, R.N.J.; Konoplev, A.V.; Kudelsky, A.V.; Madruga, M.J.; Voitsekhovitch, O.V.; Zibolt, G.

    2005-01-01

    Simplified dynamic models have been developed for predicting the concentrations of radiocesium, radiostrontium, and 131I in surface waters and freshwater fish following a large-scale radioactive fallout. The models are intended to give averaged estimates for radionuclides in water bodies and in fish

  14. Mean size among the particles of short-lived radon daughter products in the atmosphere

    International Nuclear Information System (INIS)

    Nakatani, S.

    1980-01-01

    The diffusion-battery method is used to classify the radioactive particles according to their sizes. The diffusion coefficient is determined from the fractional penetration of the particles through the battery. Particle radii are derived from the diffusion coefficients with the Stokes-Cunningham-Millikan formula. At the exit and entrance of the battery, individual concentrations of radon daughter products 218 Po, 214 Pb, 214 Bi are determined. Thus the mean sizes of individual radon daughters can be obtained from the fractional penetration of individual nuclides through the diffusion battery. Despite large statistical fluctuations the mean size of 214 Bi is always shifted toward the larger size region as compared with those of other radionuclides

  15. European roe deer antlers as an environmental archive for fallout 236U and 239Pu

    International Nuclear Information System (INIS)

    Froehlich, M.B.; Steier, P.; Wallner, G.; Fifield, L.K.

    2016-01-01

    Anthropogenic 236 U and 239 Pu were measured in European roe deer antlers hunted between 1955 and 1977 which covers and extends beyond the period of intensive nuclear weapons testing (1954–1962). The antlers were hunting trophies, and hence the hunting area, the year of shooting and the approximate age of each animal is given. Uranium and plutonium are known to deposit in skeletal tissue. Since antler histology is similar to bone, both elements were expected in antlers. Furthermore, roe deer shed their antlers annually, and hence antlers may provide a time-resolved environmental archive for fallout radionuclides. The radiochemical procedure is based on a Pu separation step by anion exchange (Dowex 1 × 8) and a subsequent U purification by extraction chromatography using UTEVA ® . The samples were measured by Accelerator Mass Spectrometry at the VERA facility (University of Vienna). In addition to the 236 U and 239 Pu concentrations, the 240 Pu/ 239 Pu isotopic ratios were determined with a mean value of 0.172 ± 0.023 which is in agreement with the ratio of global fallout (∼0.18). Rather high 236 U/ 238 U ratios of the order of 10 −6 were observed. These measured ratios, where the 236 U arises only from global fallout, have implications for the use of the 236 U/ 238 U ratio as a fingerprint for nuclear accidents or releases from nuclear facilities. Our investigations have shown the potential to use antlers as a temporally resolved archive for the uptake of actinides from the environment. - Highlights: • Roe deer antlers were studied as an environmental archive for the retrospective study of fallout isotopes 236 U and 239 Pu. • The rather high 236 U/ 238 U ratios of about 10 −6 suggest 236 U as a fingerprint tool for nuclear material releases. • The 240 Pu/ 239 Pu atom ratio underpins global fallout as the main anthropogenic contributor in antlers.

  16. Radionuclide cisternography

    International Nuclear Information System (INIS)

    Song, H.H.

    1980-01-01

    The purpose of this thesis is to show that radionuclide cisternography makes an essential contribution to the investigation of cerebrospinal fluid (CSF) dynamics, especially for the investigation of hydrocephalus. The technical details of radionuclide cisternography are discussed, followed by a description of the normal and abnormal radionuclide cisternograms. The dynamics of CFS by means of radionuclide cisternography were examined in 188 patients in whom some kind of hydrocephalus was suspected. This study included findings of anomalies associated with hydrocephalus in a number of cases, such as nasal liquorrhea, hygromas, leptomeningeal or porencephalic cysts. The investigation substantiates the value of radionuclide cisternography in the diagnosis of disturbances of CSF flow. The retrograde flow of radiopharmaceutical into the ventricular system (ventricular reflux) is an abnormal phenomenon indicating the presence of communicating hydrocephalus. (Auth.)

  17. Medical application of radionuclides and the resulting radiation exposure of parts of the population

    International Nuclear Information System (INIS)

    Keller, K.D.; Gloebel, B.; Andres, C.

    1985-01-01

    In a big hospital an investigation was made to find out to what extent the radionuclides used there contribute to the radiation exposure of the population living in the vicinity. The hospital used about 100 Ci of short-lived radionuclides a year. By applying the calculation basis stipulated by the Federal Ministry of the Interior, the radiation exposure was calculated for unfavourable cases. As a result, up to 30 mrem/a can theoretically be reached. (orig.) [de

  18. Multi-model evaluation of short-lived pollutant distributions over east Asia during summer 2008

    Science.gov (United States)

    Quennehen, B.; Raut, J.-C.; Law, K. S.; Daskalakis, N.; Ancellet, G.; Clerbaux, C.; Kim, S.-W.; Lund, M. T.; Myhre, G.; Olivié, D. J. L.; Safieddine, S.; Skeie, R. B.; Thomas, J. L.; Tsyro, S.; Bazureau, A.; Bellouin, N.; Hu, M.; Kanakidou, M.; Klimont, Z.; Kupiainen, K.; Myriokefalitakis, S.; Quaas, J.; Rumbold, S. T.; Schulz, M.; Cherian, R.; Shimizu, A.; Wang, J.; Yoon, S.-C.; Zhu, T.

    2016-08-01

    is too weak to explain the differences between the models. Our results rather point to an overestimation of SO2 emissions, in particular, close to the surface in Chinese urban areas. However, we also identify a clear underestimation of aerosol concentrations over northern India, suggesting that the rapid recent growth of emissions in India, as well as their spatial extension, is underestimated in emission inventories. Model deficiencies in the representation of pollution accumulation due to the Indian monsoon may also be playing a role. Comparison with vertical aerosol lidar measurements highlights a general underestimation of scattering aerosols in the boundary layer associated with overestimation in the free troposphere pointing to modelled aerosol lifetimes that are too long. This is likely linked to too strong vertical transport and/or insufficient deposition efficiency during transport or export from the boundary layer, rather than chemical processing (in the case of sulphate aerosols). Underestimation of sulphate in the boundary layer implies potentially large errors in simulated aerosol-cloud interactions, via impacts on boundary-layer clouds.This evaluation has important implications for accurate assessment of air pollutants on regional air quality and global climate based on global model calculations. Ideally, models should be run at higher resolution over source regions to better simulate urban-rural pollutant gradients and/or chemical regimes, and also to better resolve pollutant processing and loss by wet deposition as well as vertical transport. Discrepancies in vertical distributions require further quantification and improvement since these are a key factor in the determination of radiative forcing from short-lived pollutants.

  19. Multi-model evaluation of short-lived pollutant distributions over east Asia during summer 2008

    Directory of Open Access Journals (Sweden)

    B. Quennehen

    2016-08-01

    mitigation in Beijing is too weak to explain the differences between the models. Our results rather point to an overestimation of SO2 emissions, in particular, close to the surface in Chinese urban areas. However, we also identify a clear underestimation of aerosol concentrations over northern India, suggesting that the rapid recent growth of emissions in India, as well as their spatial extension, is underestimated in emission inventories. Model deficiencies in the representation of pollution accumulation due to the Indian monsoon may also be playing a role. Comparison with vertical aerosol lidar measurements highlights a general underestimation of scattering aerosols in the boundary layer associated with overestimation in the free troposphere pointing to modelled aerosol lifetimes that are too long. This is likely linked to too strong vertical transport and/or insufficient deposition efficiency during transport or export from the boundary layer, rather than chemical processing (in the case of sulphate aerosols. Underestimation of sulphate in the boundary layer implies potentially large errors in simulated aerosol–cloud interactions, via impacts on boundary-layer clouds.This evaluation has important implications for accurate assessment of air pollutants on regional air quality and global climate based on global model calculations. Ideally, models should be run at higher resolution over source regions to better simulate urban–rural pollutant gradients and/or chemical regimes, and also to better resolve pollutant processing and loss by wet deposition as well as vertical transport. Discrepancies in vertical distributions require further quantification and improvement since these are a key factor in the determination of radiative forcing from short-lived pollutants.

  20. Oceanic distributions of radionuclides from nuclear weapons testing

    International Nuclear Information System (INIS)

    Bowen, V.T.

    1977-01-01

    Data on the transport of fallout radionuclides in the Atlantic and Pacific Oceans are reviewed. Relevance of water column fallout data to the disposal of radioactive waste in marine locations is discussed. It is pointed out that regional patterns of delivery of soluble radionuclides must be assumed to persist at least for decades, in spite of the homogenizing action of ocean current systems and that, although there are delays in relation to density discontinuities in the water column, particle-associated radionuclides are generally delivered directly to the sediment surface. The chemistry of particle association appears increasingly complex, in relation both to the element selectivity among kinds of particles, and the stability of the associations once formed, and regional conditions may lead to retention of Pu (and possibly other nuclides) in discrete layers or throughout the water column, in opposition to its general tendency to associate with particles

  1. Transport and accumulation of radionuclides in soil

    International Nuclear Information System (INIS)

    Frissel, M.J.; Jakubick, A.T.; Kernforschungszentrum Karlsruhe G.m.b.H.

    1979-01-01

    The movement of radioactive isotopes through the water phase of soils is by far the most important. Most of the water-transported radioactive isotopes (radionuclides) occur via their dissolved salts, while the rest is carried by small soil particles to which the radionuclides are adsorbed. In the case of many chemicals, it is possible to calculate the movement or migration through soil from adsorption measurements made in the laboratory and from knowledge of the flow pattern of soil water. With increasing complexity of the chemical-soil-water system predictions become more uncertain. In the case of radionuclides the amounts expressed in units of weight are extremely small. This renders terms such as 'soluble' or 'insoluble' inapplicable. In these cases transport of 'radiocolloids' and adsorbed particles as 'insoluble' compounds may be more significant. For fallout strontium and cesium reliable predictive models have been developed. For fallout plutonium such models are under development. For calculations or predictions of the migration of radioactive material from deep soil layers to the soil surface fewer mathematical models are available. Many laboratory studies cannot yet be made due to lack of suitable soil samples from the sites under study. Nevertheless safety studies already carried out in a preliminary way are reliable, since factos such as adsorption of radionuclides on soils are neglected; consequently most safety studies overestimate possible risks. Further studies are required to ascertain how 'pessimistic' are the present safety criteriy. (orig./MG) [de

  2. Radionuclides in air, water, and biota

    International Nuclear Information System (INIS)

    Seymour, A.H.; Nelson, V.A.

    1977-01-01

    Air, water, and biological samples collected before and after the 1965, 1969, and 1971 underground nuclear detonations at Amchitka Island were analyzed for natural and fallout radionuclides by gamma spectrometry. Selected samples were also analyzed for tritium, 55 Fe, and 90 Sr. The objectives were to search for and identify radionuclides of Amchitka origin in the samples and to contribute to the general knowledge of the distribution of radionuclides in the environment. The studies showed that there has been no escape of radionuclides from the underground sites of the three nuclear detonations at Amchitka Island except for trace quantities of radionuclides, principally tritium, in water and soil gas samples from the immediate vicinity of the surface ground zero for the 1965 event. Two naturally occurring radionuclides, 40 K and 7 Be, were the most abundant radionuclides in the samples, usually by a factor of 10 or more, except for 137 Cs in lichen samples. All levels were well below applicable Radiation Protction Guides, often being near the statistical limit of detection

  3. Determination of Fallout Radionuclides in Environmental Samples by Gamma-Ray Spectrometry; Mesure Spectrometrique Gamma des Radionucleides de Retombee Presents dans des Echantillons du Millieu; Opredelenie radioizotopov radioaktivnykh osadkov v probakh iz okruzhayushchej sredy pri pomoshchi spektrometrii gamma-luchej; Determinacion, por Espectrometria Gamma, de los Radionuclidos de Precipitaciones en Muestras del Medio Ambiente

    Energy Technology Data Exchange (ETDEWEB)

    Ward, G. M.; Johnson, J. E.; Wilson, D. W. [Department of Animal Science, Colorado State University, Fort Collins, CO (United States)

    1965-10-15

    NaOH (fallout {sup 137}Cs is completely soluble only in strong bases) and filtering, which removes about 93% of the Zr-{sup 95}Nb. Elution of rainwater concentrate from columns with 1 M MN{sub 4}NO{sub 3}; quantitatively removed {sup 137}Cs and effectively separated the Zr-{sup 95}Nb and {sup 54}Mn activity. When all the photopeaks were apparent, either by decay or chemical separation, quantitative estimation of each radionuclide was possible by calibration with each nuclide and calculation of the Compton effects of each. The resultant equations were solved with an IBM 1620 computer and a programme prepared to solve for the concentration of each of the nine nuclides mentioned above. The same programme was used to solve for {sup 137}Cs and {sup 40}K content of milk, meat and Urine, which is simpler and the errors are smaller. (author) [French] Depuis mai 1962, de nombreux echantillons du milieu sont recueillis sur la ferme de l'Universite, pour etudier le passage de {sup 137}Cs a travers une partie importante de la chaine alimentaire de l'homme. Tous les echantillons mesures avaient une faible activite specifique et les mesures ont ete faites avec un ensemble spectrometrique pour rayons gamma de faible energie, muni d'un cristal Nal(Tl) de 20 cm de diametre et de 10 cm d'epaisseur protege contre le mouvement propre par une chambre a parois d'acier de 12,5 cm d'epaisseur et branche sur un analyseur d'amplitude a 400 canaux. Les auteurs ont procede au comptage direct, selon une geometrie constante de tampons de filtres a air, d'importants echantillons (1 kg) de fourrages, de cereales et de bouse seches. Ils ont concentre des echantillons de precipitations en les faisant passer dans des colonnes d'echange de cations Dowex-50. Le lait, la viande et l'urine ont ete places pour le comptage dans de grands recipients annulaires en lucite. Les seuls radionuclides emetteurs gamma trouves dans ces matieres sont {sup 137}Cs, {sup 40}K, {sup 131}I et {sup 141}0 Ba-La; ils sont en

  4. Temporary/portable nuclear fallout shelter

    Energy Technology Data Exchange (ETDEWEB)

    Hampel, V E

    1991-01-15

    The design and invention of a temporary/portable fallout shelter has been described in context of schematic and representative embodiments. Tent structures are described which include disposable, exterior, semi-transparent plastic and/or fabric shield membranes covering a tent composed of stretched, tightly woven, rip-resistant fabric panels supported by tensile rods/wands. 16 figs.

  5. Dosimetric substantiation of the use of radionuclide methods in obstetrics

    International Nuclear Information System (INIS)

    Volobuev, A.I.; Filatov, V.I.; Turaev, R.N.

    1987-01-01

    The problem of a possible use of radionuclide methods of investigation (placentography and renography) in obstetrics was considered. Doses and permissibles activities in pregnant women of the AP category belonging to groups at high risk of obstetric and perinated pathology were worked out on the basis of the ''Rules and standards of open radiopharmaceuticals in diagnostic purposes'' (1984). The above investigations using the administration of short-lived radionuclides with total activity of 7.4 MBq ( 99m Tc-albumin and DTPA) were shown to be safe for mother and fetus

  6. Contributions of short-lived radioiodines to thyroid doses received by evacuees from the Chernobyl area estimated using early in vivo activity measurements

    International Nuclear Information System (INIS)

    Balonov, M.; Kaidanovsky, G.; Zvonova, I.; Kovtun, A.; Bouville, A.; Luckyanov, L.; Voilleque, P.

    2003-01-01

    A series of in-vivo gamma spectrometric measurements of 65 people, evacuated from Pripyat 1.5 days after the Chernobyl Nuclear Power Plant Unit 4 explosion was performed in St. Petersburg, Russia, as early as 30 April 1986. The historical spectra and interviews were recently processed and the results used for thyroid dose estimation. Activities of 131 I in thyroid and 132 Te in lungs were determined easily; for estimation of 132 I and 133 I activities in thyroid, sophisticated methods of spectra processing were developed. According to thyroid measurement data, the mean ratio of 133 I/ 131 I activities (at the time of the accident) inhaled by residents of Pripyat was 2.0. The mean ratio of thyroid dose from 133 I inhalation to that caused by 131 I amounts to 0.3, which confirms accuracy of dose estimates based on the evolution of the Chernobyl accident. The mean ratio of 132 I activity in thyroid to that of 132 Te in lungs was assessed from the human measurement data to be 0.2, which is in reasonable agreement with the metabolic properties of these radionuclides. The mean ratio of thyroid dose from 132 I originating from 132 Te deposited in lungs to the dose caused by 131 I was 0.13 ± 0.02 for Pripyat residents who did not take KI pills and 0.9 ± 0.1 for persons who took KI pills. Thus, the contribution of short-lived radioiodines to total thyroid dose of Pripyat residents, which was on average 30% for persons who did not apply stable iodine prophylaxis, and about 50% for persons who took KI pills on 26-27 April, should be accounted for in the assessment of thyroid health effects. (author)

  7. The medical effects of radioactive fall-out: role of stable end-products

    International Nuclear Information System (INIS)

    Burrows, B.A.; Cardarelli, J.C.; Boling, E.A.; Sinex, F.M.

    1980-01-01

    To summarize, from preliminary observations on the possible effects of radioactive fall-out, it may be inferred that in addition to the secondary products of ionizing irradiation per se, the stable end-products of the transmutation of certain radionuclides may adversely influence cellular metabolism, including mutagenesis. The discussion of the possible role of intracellular barium as an end-product of 137Cs decay is offered as an example of an unpredictable number of broad ecological, as well as the more limited medical, effects that may be of both clinical and climatological significance

  8. The transfer of fallout cesium-137 from browse to moose. Part 1

    International Nuclear Information System (INIS)

    Zach, R.; Mayoh, K.R.

    1982-09-01

    We are investigating the transfer of fallout cesium-137 from soil to browse to moose (Alces alces) to wolf (Canis lupis) to promote our understanding of the movement of radionuclides through natural food chains. The first part of this study is concerned with moose food habits. Early winter food habits of moose from Hecla Island and Manitoba Game Hunting Area 26 in south central and south eastern Manitoba were studied. In 86 rumen samples, 25 food types were identified. Three methods of food habit determination were used: (1) percentage occurrence of food types, (2) subjective abundance scores and (3) percentage dry weight. All three methods yielded very similar results

  9. Contamination dynamics in fallouts, pasturable vegetation and milk in Leningrad distrist after Chernobyl accident

    International Nuclear Information System (INIS)

    Nedbaevskaya, N.A.; Sanzharova, N.I.; Blinova, L.D.; Kryshev, I.I.; Aleksakhin, R.M.

    1991-01-01

    Radiation monitoring of individual elements of agroecosystem in the area of the Leningrad NPP is carried out with the purpose of studying the concentration dynamics of radioisotopes in the atmosphere resulting from the accident at the Chernobyl NPP. The γ-radiation dose rate on the terrain, content and radionuclide composition of atmospheric fallout, content of γ-emitting isotopes in the soil and plants at pastures is monitored from April up to September 1986; radioisotope content in cow milk by pasturing is determined

  10. Determination of radionuclide concentrations in animal feedstuffs for use following a nuclear emergency

    International Nuclear Information System (INIS)

    Hwang, W. T.; Ser, K. S.; Kim, E. H.; Choi, Y. K.; Han, M. H.; Choi, Y. H.

    2001-01-01

    The optimized derived intervention levels for animal products were evaluated based on cost-benefit analysis. From these results, the radionuclide concentrations in animal feedstuffs for use were derived. It was shown that radionuclide concentrations in animal feedstuffs for use depend strongly on animal products, radionuclides and feeding period. In case of the contaminated feedstuffs with long-lived radionuclides ( 137 Cs, 90 Sr), the feedstuffs with lower contamination should be supplied to animals with increase of feeding period due to the accumulation of radionuclides in animal products. While, in case of the contaminated feedstuffs with short-lived radionuclides ( 131 I), the feeding of higher contaminated feedstuffs was possible with increase of feeding period due to radionuclide decay. It was shown that 137 Cs concentration was lower than 90 Sr concentration in animal feedstuffs for use. It is primarily due to the higher feed-animal products transfer factor of 137 Cs

  11. Activity concentration of radionuclides in plants in the environment of western Ghats

    International Nuclear Information System (INIS)

    Manigandan, P. K.

    2009-01-01

    A field study on the transfer of primordial radionuclides 238 U, 232 Th, 40 K and fallout radionuclides 210 Po in different plant species in tropical forest of western Ghats environment is presented. Material and Methods: The Top storey, Second storey, Shrubs and epiphytic plant species were chosen and concentration of these radionuclides in plant and soil were measured by employing gamma ray spectrometer and alpha counter. Results: The concentration ratio shows the variation in different species while a wild plant Elaeocarpus oblongus and epiphytic plants indicated preferential uptake of these radionuclides. Conclusion: The dust trapped in the root system of. epiphytic plants could be used as bio indicator to monitor fallout radionuclides in the Western Ghats. The concentration of 232 Th and 40 K in leaves depends on the age of the leaves.

  12. The behaviour of radionuclides in soil

    International Nuclear Information System (INIS)

    Bunzl, K.

    1987-01-01

    Radionuclides in soil are of natural as well as of artificial origin. Their migration in the soil and their availability for ecological processes depend considerably on the extent at which they are sorbed. The methods for the determination of the vertical rate of migration are described. For most radionuclides this transport is very slow (a few cm per year). Cs-137 is of especial interest. It is sorbed strongly by most soils and, as a consequence, its root uptake is small. However, as a result of the sorption, this radionuclide is eluted from the root zone only very slowly and its thus available for the root uptake for many years. The Cs-137 concentrations in plants to be expected in the coming years as a result of the fallout from Chernobyl are small. (orig.) [de

  13. Radionuclide carrier

    International Nuclear Information System (INIS)

    Hartman, F.A.; Kretschmar, H.C.; Tofe, A.J.

    1978-01-01

    A physiologically acceptable particulate radionuclide carrier is described. It comprises a modified anionic starch derivative with 0.1% to 1.5% by weight of a reducing agent and 1 to 20% by weight of anionic substituents

  14. Centuries of thermal sea-level rise due to anthropogenic emissions of short-lived greenhouse gases.

    Science.gov (United States)

    Zickfeld, Kirsten; Solomon, Susan; Gilford, Daniel M

    2017-01-24

    Mitigation of anthropogenic greenhouse gases with short lifetimes (order of a year to decades) can contribute to limiting warming, but less attention has been paid to their impacts on longer-term sea-level rise. We show that short-lived greenhouse gases contribute to sea-level rise through thermal expansion (TSLR) over much longer time scales than their atmospheric lifetimes. For example, at least half of the TSLR due to increases in methane is expected to remain present for more than 200 y, even if anthropogenic emissions cease altogether, despite the 10-y atmospheric lifetime of this gas. Chlorofluorocarbons and hydrochlorofluorocarbons have already been phased out under the Montreal Protocol due to concerns about ozone depletion and provide an illustration of how emission reductions avoid multiple centuries of future TSLR. We examine the "world avoided" by the Montreal Protocol by showing that if these gases had instead been eliminated in 2050, additional TSLR of up to about 14 cm would be expected in the 21st century, with continuing contributions lasting more than 500 y. Emissions of the hydrofluorocarbon substitutes in the next half-century would also contribute to centuries of future TSLR. Consideration of the time scales of reversibility of TSLR due to short-lived substances provides insights into physical processes: sea-level rise is often assumed to follow air temperature, but this assumption holds only for TSLR when temperatures are increasing. We present a more complete formulation that is accurate even when atmospheric temperatures are stable or decreasing due to reductions in short-lived gases or net radiative forcing.

  15. Development of a Method to Assess the Radiation Dose due to Internal Exposure to Short-lived Radioactive Materials

    International Nuclear Information System (INIS)

    Benmaman, D.; Koch, J.; Ribak, J.

    2014-01-01

    Work with radioactive materials requires monitoring of the employees' exposure to ionizing radiation. Employees may be exposed to radiation from internal and/or external exposure. Control of external exposure is mostly conducted through personal radiation dosimeters provided to employees. Control of internal exposure can be performed by measuring the concentration of radioactive substances excreted in urine or through whole-body counting in which the entire body or target organs are scanned with a sensitive detector system (1). According to the regulations in Israel an employee that may be internally exposed must undergo an exposure control at least once every three months. The idea lying behind the control of internal exposure by urine testing is that if radioactive material has penetrated into the employee body, it can be detected even if the test is performed once every three months. A model was fitted for each element describing its dispersion in the body and its excretion therefrom (2). By means of this model, one can estimate the activity that entered the body and calculate the resulting radiation dose to which the worker was exposed. There is a problem to implement this method when it comes to short-lived radioactive materials, for which it is very likely that the material that penetrated into the body has decayed and cannot be detected by testing once every three months. As a result, workers with short-lived radioactive materials are presently not monitored for internal exposure, in contradiction to the requirements of the Safety at Work Regulations. The purpose of the study is to develop an alternative method to assess the amount of radioactive material absorbed in the body and the resulting radiation dose due to internal exposure of workers to short-lived radioactive materials

  16. Online selection of short-lived particles on many-core computer architectures in the CBM experiment at FAIR

    Energy Technology Data Exchange (ETDEWEB)

    Zyzak, Maksym

    2016-07-07

    Modern experiments in heavy ion collisions operate with huge data rates that can not be fully stored on the currently available storage devices. Therefore the data flow should be reduced by selecting those collisions that potentially carry the information of the physics interest. The future CBM experiment will have no simple criteria for selecting such collisions and requires the full online reconstruction of the collision topology including reconstruction of short-lived particles. In this work the KF Particle Finder package for online reconstruction and selection of short-lived particles is proposed and developed. It reconstructs more than 70 decays, covering signals from all the physics cases of the CBM experiment: strange particles, strange resonances, hypernuclei, low mass vector mesons, charmonium, and open-charm particles. The package is based on the Kalman filter method providing a full set of the particle parameters together with their errors including position, momentum, mass, energy, lifetime, etc. It shows a high quality of the reconstructed particles, high efficiencies, and high signal to background ratios. The KF Particle Finder is extremely fast for achieving the reconstruction speed of 1.5 ms per minimum-bias AuAu collision at 25 AGeV beam energy on single CPU core. It is fully vectorized and parallelized and shows a strong linear scalability on the many-core architectures of up to 80 cores. It also scales within the First Level Event Selection package on the many-core clusters up to 3200 cores. The developed KF Particle Finder package is a universal platform for short- lived particle reconstruction, physics analysis and online selection.

  17. Online selection of short-lived particles on many-core computer architectures in the CBM experiment at FAIR

    International Nuclear Information System (INIS)

    Zyzak, Maksym

    2016-01-01

    Modern experiments in heavy ion collisions operate with huge data rates that can not be fully stored on the currently available storage devices. Therefore the data flow should be reduced by selecting those collisions that potentially carry the information of the physics interest. The future CBM experiment will have no simple criteria for selecting such collisions and requires the full online reconstruction of the collision topology including reconstruction of short-lived particles. In this work the KF Particle Finder package for online reconstruction and selection of short-lived particles is proposed and developed. It reconstructs more than 70 decays, covering signals from all the physics cases of the CBM experiment: strange particles, strange resonances, hypernuclei, low mass vector mesons, charmonium, and open-charm particles. The package is based on the Kalman filter method providing a full set of the particle parameters together with their errors including position, momentum, mass, energy, lifetime, etc. It shows a high quality of the reconstructed particles, high efficiencies, and high signal to background ratios. The KF Particle Finder is extremely fast for achieving the reconstruction speed of 1.5 ms per minimum-bias AuAu collision at 25 AGeV beam energy on single CPU core. It is fully vectorized and parallelized and shows a strong linear scalability on the many-core architectures of up to 80 cores. It also scales within the First Level Event Selection package on the many-core clusters up to 3200 cores. The developed KF Particle Finder package is a universal platform for short- lived particle reconstruction, physics analysis and online selection.

  18. Harvard-MIT research program in short-lived radiopharmaceuticals. Progress report, March 1, 1985-February 28, 1986

    International Nuclear Information System (INIS)

    1986-03-01

    The Harvard-MIT Research Program in Short-Lived Radiopharmaceuticals was established in 1977 to foster interaction among groups working at Harvard Medical School, the Massachusetts Institute of Technology and the Massachusetts General Hospital in fields related to radiopharmaceutical chemistry. From these collaborations and building upon the special, but different, strengths of the participating individuals, laboratories and institutions, it was hoped that original approaches would be found for the design of new, clinically useful, labeled compounds. We believe that examination of the record demonstrates that this has been a fruitful alliance

  19. Harvard-MIT research program in short-lived radiopharmaceuticals. Progress report, March 1, 1983-February 29, 1984

    International Nuclear Information System (INIS)

    Adelstein, S.J.; Brownell, G.L.

    1984-02-01

    This report describes research efforts towards the achievement of a clearer understanding of the solution chemistry of technetium in order to facilitate the design of future clinical agents labeled with Tc-99m, the development of new receptor binding radiopharmaceuticals for the in vivo assessment of insulin receptors and for imaging the adrenal medulla and the brain, the examination of the utility of monoclonal antibodies and liposomes in the design of radiopharmaceuticals for diagnosis and therapy, and the synthesis of short-lived positron-emitting radiopharmaceuticals for transverse imaging of regional physiological processes

  20. Large drainages from short-lived glacial lakes in the Teskey Range, Tien Shan Mountains, Central Asia

    Science.gov (United States)

    Narama, Chiyuki; Daiyrov, Mirlan; Duishonakunov, Murataly; Tadono, Takeo; Sato, Hayato; Kääb, Andreas; Ukita, Jinro; Abdrakhmatov, Kanatbek

    2018-04-01

    Four large drainages from glacial lakes occurred during 2006-2014 in the western Teskey Range, Kyrgyzstan. These floods caused extensive damage, killing people and livestock as well as destroying property and crops. Using satellite data analysis and field surveys of this area, we find that the water volume that drained at Kashkasuu glacial lake in 2006 was 194 000 m3, at western Zyndan lake in 2008 was 437 000 m3, at Jeruy lake in 2013 was 182 000 m3, and at Karateke lake in 2014 was 123 000 m3. Due to their subsurface outlet, we refer to these short-lived glacial lakes as the tunnel-type, a type that drastically grows and drains over a few months. From spring to early summer, these lakes either appear, or in some cases, significantly expand from an existing lake (but non-stationary), and then drain during summer. Our field surveys show that the short-lived lakes form when an ice tunnel through a debris landform gets blocked. The blocking is caused either by the freezing of stored water inside the tunnel during winter or by the collapse of ice and debris around the ice tunnel. The draining then occurs through an opened ice tunnel during summer. The growth-drain cycle can repeat when the ice-tunnel closure behaves like that of typical supraglacial lakes on debris-covered glaciers. We argue here that the geomorphological characteristics under which such short-lived glacial lakes appear are (i) a debris landform containing ice (ice-cored moraine complex), (ii) a depression with water supply on a debris landform as a potential lake basin, and (iii) no visible surface outflow channel from the depression, indicating the existence of an ice tunnel. Applying these characteristics, we examine 60 depressions (> 0.01 km2) in the study region and identify here 53 of them that may become short-lived glacial lakes, with 34 of these having a potential drainage exceeding 10 m3 s-1 at peak discharge.

  1. Large drainages from short-lived glacial lakes in the Teskey Range, Tien Shan Mountains, Central Asia

    Directory of Open Access Journals (Sweden)

    C. Narama

    2018-04-01

    Full Text Available Four large drainages from glacial lakes occurred during 2006–2014 in the western Teskey Range, Kyrgyzstan. These floods caused extensive damage, killing people and livestock as well as destroying property and crops. Using satellite data analysis and field surveys of this area, we find that the water volume that drained at Kashkasuu glacial lake in 2006 was 194 000  m3, at western Zyndan lake in 2008 was 437 000 m3, at Jeruy lake in 2013 was 182 000 m3, and at Karateke lake in 2014 was 123 000 m3. Due to their subsurface outlet, we refer to these short-lived glacial lakes as the tunnel-type, a type that drastically grows and drains over a few months. From spring to early summer, these lakes either appear, or in some cases, significantly expand from an existing lake (but non-stationary, and then drain during summer. Our field surveys show that the short-lived lakes form when an ice tunnel through a debris landform gets blocked. The blocking is caused either by the freezing of stored water inside the tunnel during winter or by the collapse of ice and debris around the ice tunnel. The draining then occurs through an opened ice tunnel during summer. The growth–drain cycle can repeat when the ice-tunnel closure behaves like that of typical supraglacial lakes on debris-covered glaciers. We argue here that the geomorphological characteristics under which such short-lived glacial lakes appear are (i a debris landform containing ice (ice-cored moraine complex, (ii a depression with water supply on a debris landform as a potential lake basin, and (iii no visible surface outflow channel from the depression, indicating the existence of an ice tunnel. Applying these characteristics, we examine 60 depressions (> 0.01 km2 in the study region and identify here 53 of them that may become short-lived glacial lakes, with 34 of these having a potential drainage exceeding 10 m3 s−1 at peak discharge.

  2. The low to intermediate activity and short living waste storage facility. For a controlled management of radioactive wastes

    International Nuclear Information System (INIS)

    2006-01-01

    Sited at about 50 km of Troyes (France), the Aube facility started in 1992 and has taken over the Manche facility for the surface storage of low to intermediate and short living radioactive wastes. The Aube facility (named CSFMA) is the answer to the safe management of these wastes at the industrial scale and for 50 years onward. This brochure presents the facility specifications, the wastes stored at the center, the surface storage concept, the processing and conditioning of waste packages, and the environmental monitoring performed in the vicinity of the site. (J.S.)

  3. Impact of preindustrial to present-day changes in short-lived pollutant emissions on atmospheric composition and climate forcing

    Science.gov (United States)

    Naik, Vaishali; Horowitz, Larry W.; Fiore, Arlene M.; Ginoux, Paul; Mao, Jingqiu; Aghedo, Adetutu M.; Levy, Hiram

    2013-07-01

    We describe and evaluate atmospheric chemistry in the newly developed Geophysical Fluid Dynamics Laboratory chemistry-climate model (GFDL AM3) and apply it to investigate the net impact of preindustrial (PI) to present (PD) changes in short-lived pollutant emissions (ozone precursors, sulfur dioxide, and carbonaceous aerosols) and methane concentration on atmospheric composition and climate forcing. The inclusion of online troposphere-stratosphere interactions, gas-aerosol chemistry, and aerosol-cloud interactions (including direct and indirect aerosol radiative effects) in AM3 enables a more complete representation of interactions among short-lived species, and thus their net climate impact, than was considered in previous climate assessments. The base AM3 simulation, driven with observed sea surface temperature (SST) and sea ice cover (SIC) over the period 1981-2007, generally reproduces the observed mean magnitude, spatial distribution, and seasonal cycle of tropospheric ozone and carbon monoxide. The global mean aerosol optical depth in our base simulation is within 5% of satellite measurements over the 1982-2006 time period. We conduct a pair of simulations in which only the short-lived pollutant emissions and methane concentrations are changed from PI (1860) to PD (2000) levels (i.e., SST, SIC, greenhouse gases, and ozone-depleting substances are held at PD levels). From the PI to PD, we find that changes in short-lived pollutant emissions and methane have caused the tropospheric ozone burden to increase by 39% and the global burdens of sulfate, black carbon, and organic carbon to increase by factors of 3, 2.4, and 1.4, respectively. Tropospheric hydroxyl concentration decreases by 7%, showing that increases in OH sinks (methane, carbon monoxide, nonmethane volatile organic compounds, and sulfur dioxide) dominate over sources (ozone and nitrogen oxides) in the model. Combined changes in tropospheric ozone and aerosols cause a net negative top

  4. Application of dynamic and transition magnetic fields for determination of magnetic moments of short-lived nuclear states

    International Nuclear Information System (INIS)

    Burgov, N.A.

    1986-01-01

    Problem of measuring magnetic momenta of short-living nuclear states is discussed. Different methods for measuring magnetic momenta using interionic and transient magnetic fields were considered. Possibility for determining a value g by means of measuring correlation attenuation is investigated as well as measuring magnetic momenta by means of inclined foils. At present 2 + level magnetic momenta for many odd-odd nuclei have been determined by means of the above methods. The methods are only ones for determining magnetic momenta of nuclear levels with small lifetimes up to tenth and hundredth of shares of picoseconds

  5. Radionuclide cycling in a Utah dairy farm

    International Nuclear Information System (INIS)

    Thomas, J.M.; Eberhardt, L.L.; Hawthorne, H.A.; Zellmer, S.D.

    1976-01-01

    Both detailed and summarized data are presented for 137 Cs and for 90 Sr which resulted from a study of the deposition of fallout radionuclides into a Utah dairy farm. In addition, mathematical models and statistical methods (including nonlinear least-squares techniques) were used to obtain estimates of key parameters for a compartmental model of the dynamics of 137 Cs transfers in the dairy system. Both the results of laboratory studies and field observations were used to derive the estimates and to construct functional relationships for the model. Two computer models were used to further analyze and evaluate consistency of the fallout-alfalfa-milk sequence of data. The results of this study are compared with two similar investigations (in Colorado and Michigan) and are used to examine earlier analyses of the general system studied. Extensive data tabulations are also presented

  6. The results of artificial radionuclides monitoring in the Baltic sea

    International Nuclear Information System (INIS)

    Astrauskiene, N.; Lukinskiene, M; Zemaitiene, G.

    1994-01-01

    Long-term radionuclides volume activity (v.a.) monitoring (1976-1990) data showed that measurement results obtained in steady observation station give reliable information of the coastal area of the Baltic sea radioactive equilibrium between atmosphere and surface water was observed in the coastal zone. Chernobyl Power Plant accident influenced upon the Baltic sea coastal water by radionuclides 137 Cs and 144 Ce. Radionuclide 90 Sr volume activity was practically unchangerable. The mechanism of radionuclides fallout from atmosphere are various. lt can be illustrated by 137 Cs and 144 Ce a.v. structure field variations in open sea and coastal zone near Juodkrante. The Baltic sea inhomogeneous contamination by radionuclide 137 Cs in 1988-1990 leads to equalization of 137 Cs v.a. in the surface waters and it causes v.a. increase in coastal waters. (author)

  7. Latitudinal distribution of cesium-137 fallout in 1990 on Saxifraga oppositofolia from Ellesmere Island, Canada

    International Nuclear Information System (INIS)

    France, R.L.; Svoboda, J.; Taylor, H.W.

    1993-01-01

    During the first ski traverse of Ellesmere Island in spring 1990, purple saxifrage (Saxifraga oppositifolia) was collected at 10 sites from 76 to 82 degrees N. Measured 137 Cs levels in this cushion plant displayed a progressive decrease in activity north of 78 degrees, reflecting past global patterns of radionuclide fallout. Lower 137 Cs activity at the southern end of Ellesmere Island may reflect a northward shift of the distribution maximum since a previous latitudinal survey conducted in 1979-1980. Levels of 137 in three species of lichen were consistently higher than those for nearby saxifrage, possibly owing to the larger exposure to fallout for much of the year and the slower rate of lichen growth. In support of previous research, no 134 Cs was detected, which indicated that Chernobyl fallout had not been deposited in significant quantities at these extreme northern latitudes. Specific activities in 1990 of saxifrage samples were compared with similar samples collected during 1979-1980 to derive an effective half-life of 6.2 ± 1.0 years for northern Ellesmere Island

  8. Reconstruction and analysis of 137Cs fallout deposition patterns in the Marshall Islands.

    Science.gov (United States)

    Whitcomb, Robert C

    2002-03-01

    Estimates of 137Cs deposition caused by fallout originating from nuclear weapons testing in the Marshall Islands have been estimated for several locations in the Marshall Islands. These retrospective estimates are based primarily on historical exposure rate and gummed film measurements. The methods used to reconstruct these deposition estimates are similar to those used in the National Cancer Institute study for reconstructing 131I deposition from the Nevada Test Site. Reconstructed cumulative deposition estimates are validated against contemporary measurements of 137Cs concentration in soil with account taken for estimated global fallout contributions. These validations show that the overall geometric bias in predicted-to-observed (P:O) ratios is 1.0 (indicating excellent agreement). The 5th to 95th percentile range of this distribution is 0.35-2.95. The P:O ratios for estimates using historical gummed film measurements tend to slightly overpredict more than estimates using exposure rate measurements. The deposition estimate methods, supported by the agreement between estimates and measurements, suggest that these methods can be used with confidence for other weapons testing fallout radionuclides.

  9. Fallout exposure and thyroid diseases prevalence in the Semipalatinsk region of Kazakhstan

    International Nuclear Information System (INIS)

    Zhumadilov, Z.S.; Bhattarcharjee, Deborshi; Abisheva, G.

    2004-01-01

    The thyroid gland is considered to be especially susceptible to nuclear fallout because radioactive isotopes of iodine, and 131 I in particular, are major components of the fallout. During the 40 year period from 1949 to 1989, at Semipalatinsk Nuclear Test Site (SNTS) near the Semipalatinsk city, 30 surface, 88 atmospheric and 340 underground explosions of nuclear and thermonuclear devices were conducted by the former Soviet Union. The radionuclides emanating from these tests resulted in atmospheric and environmental contamination in the region of Semipalatinsk and parts of region of north-eastern Kazakhstan leading to various levels of acute and chronic radiation exposure. The radiation dosimetry results revealed that external dose to the population around Semipalatinsk due to radioactive cloud and fallout from the SNTS ranged from 35cGy-100cGy. The possible relationships between radiation exposure and the prevalence of thyroid gland abnormalities around the Semipalatinsk nuclear test site area are not well established and hence a detailed study of the same is suggested

  10. Determination of k0-factors of short-lived nuclides and application of k0-NAA to selected trace elements

    International Nuclear Information System (INIS)

    Acharya, R.; Holzbecher, J.; Chatt, A.

    2012-01-01

    As part of the standardization program of k 0 -based NAA (k 0 -NAA) methods at the Dalhousie University SLOWPOKE-2 reactor (DUSR) facility, the k 0 -factors of 15 analytically important short-lived nuclides (half-life 197 Au). The elemental standards used were prepared mostly from their primary standard solutions. The samples were irradiated in both inner and outer pneumatic sites of the DUSR facility and counted using an HPGe-detector coupled to an ORTEC’s digital gamma-ray spectrometer. The k 0 -factors determined using both inner and outer irradiation sites were found to be within ±5% with respect to either recommended or literature values in most cases. The Z-score values at 95% confidence level were found to be in the range of ±0.03–1.6. The k 0 -NAA method was applied to three different NIST standard reference materials (SRMs) and concentrations of six elements, namely Ag, F, Hf, Rb, Sc, and Se were determined using their short-lived nuclides. The concentrations of these elements were also determined by relative NAA method for comparison purposes.

  11. Radionuclide data

    International Nuclear Information System (INIS)

    Anon.

    1992-01-01

    Chapter 8 presents tables on selected alpha, beta, gamma and x-ray emitters by increasing energy; information on specific activity for selected radionuclides; naturally occurring radionuclides; the natural decay series; and the artificially produced neptunium series. A table of alpha emitters is listed by increasing atomic number and by energy. The table of β emitters presented is useful in identifying β emitters whose energies and possibly half-lives have been determined by standard laboratory techniques. It is also a handy guide to β-emitting isotopes for applications requiring specific half-lives and/or energies. Gamma rays for radionuclides of importance to radiological assessments and radiation protection are listed by increasing energy. The energies and branching ratios are important for radionuclide determinations with gamma spectrometry detectors. This section also presents a table of x-ray energies which are useful for radiochemical analyses. A number of nuclides emit x-rays as part of their decay scheme. These x-rays may be counted with Ar proportional counters, Ge planar or n-type Ge co-axial detectors, or thin crystal NaI(T1) scintillation counters. In both cases, spectral measurements can be made and both qualitative and quantitative information obtained on the sample. Nuclear decay data (energy and probability by radiation type) for more than one hundred radionuclides that are important to health physicists are presented in a schematic manner

  12. Carborne fallout mapping - STUK/HUT team

    Energy Technology Data Exchange (ETDEWEB)

    Honkamaa, T.; Tiilikainen, H. [Finnish Centre for Radiation and Nuclear Safety, Helsinki (Finland); Aarnio, P.; Nikkinen, M. [Helsinki Univ. of Technology, Espoo (Finland)

    1997-12-31

    During the summer 1995 altogether 8,625 spectrometric and 3,108 dose-rate measurements were performed in Padasjoki Auttoinen village using carborne measuring devices. As a result {sup 137}Cs fallout and dose-rate maps were produced. The highest measured values in the test area II were 160 kBq m{sup -2} for fallout and 0.22 {mu}Sv h{sup -1} for dose-rate. One hot spot was found beside the test area (dose rate 0.31 {mu}Sv h{sup -1}). On the cultivated areas the measured count rates in {sup 137}Cs-window are three to four times lower than in the forest areas in average, indicating an altered depth profile of caesium. (au).

  13. FALLOUT RADIATION: EFFECTS ON THE SKIN

    Energy Technology Data Exchange (ETDEWEB)

    Conard, R. A.; Cronkite, E. P.; Bond, V. P.

    1963-02-06

    Until recently it has been generally assumed that injury to the skin from ionizing radiation was not a serious hazard associated with the detonation of nuclear dcvices. However, in 1954 the importance of this hazard became apparent when widespread lesions of the skin developed in a large group of people accidentally exposed to fallout radiation in the Marshall Islands following the experimental detonation of a large nuclear device. The accident in the Marshall Islands affords an example of large numbers of lesions of the skin in human beings from the fallout. Studies have been documented and will be referred to frequently in this chapter. The possibility of such accidents must be considered seriously in view of the increasingly widespread use of radioisotopes.

  14. Carborne fallout mapping - STUK/HUT team

    International Nuclear Information System (INIS)

    Honkamaa, T.; Tiilikainen, H.; Aarnio, P.; Nikkinen, M.

    1997-01-01

    During the summer 1995 altogether 8,625 spectrometric and 3,108 dose-rate measurements were performed in Padasjoki Auttoinen village using carborne measuring devices. As a result 137 Cs fallout and dose-rate maps were produced. The highest measured values in the test area II were 160 kBq m -2 for fallout and 0.22 μSv h -1 for dose-rate. One hot spot was found beside the test area (dose rate 0.31 μSv h -1 ). On the cultivated areas the measured count rates in 137 Cs-window are three to four times lower than in the forest areas in average, indicating an altered depth profile of caesium. (au)

  15. Modeling Fallout of Anthropogenic I-129

    DEFF Research Database (Denmark)

    Englund, Edvard; Aldahan, Als; Possnert, Göran

    2008-01-01

    Despite the relatively well-recognized emission rates of the anthropogenic 1291, there is little knowledge about the temporal fallout patterns and magnitude of fluxes since the start of the atomic era at the early 1940s. We here present measurements of annual 1291 concentrations in sediment......, a numerical model approach was used taking into account the emission rates/estimated fallout, transport pathways, and the sediment system. The model outcomes suggest a relatively dominating marine source of 1291 to north Europe compared to direct gaseous releases. A transfer rate of 1291 from sea...... to atmosphere is derived for pertinent sea areas (English Channel, Irish Sea, and North Sea), which is estimated at 0.04 to 0.21 y(-1)....

  16. Carborne fallout mapping - STUK/HUT team

    Energy Technology Data Exchange (ETDEWEB)

    Honkamaa, T; Tiilikainen, H [Finnish Centre for Radiation and Nuclear Safety, Helsinki (Finland); Aarnio, P; Nikkinen, M [Helsinki Univ. of Technology, Espoo (Finland)

    1998-12-31

    During the summer 1995 altogether 8,625 spectrometric and 3,108 dose-rate measurements were performed in Padasjoki Auttoinen village using carborne measuring devices. As a result {sup 137}Cs fallout and dose-rate maps were produced. The highest measured values in the test area II were 160 kBq m{sup -2} for fallout and 0.22 {mu}Sv h{sup -1} for dose-rate. One hot spot was found beside the test area (dose rate 0.31 {mu}Sv h{sup -1}). On the cultivated areas the measured count rates in {sup 137}Cs-window are three to four times lower than in the forest areas in average, indicating an altered depth profile of caesium. (au).

  17. Radioactive fallout in Norway in 1964

    International Nuclear Information System (INIS)

    Oftedal, P.

    1989-01-01

    Scholastic achievement of Norwegian children born in 1965 has been analysed in relation to date of birth and school address, in order to examine a possible effect of radioactive fallout during their fetal period. The Western regions of the country had an order of magnitude higher fallout contamination than the Eastern region. There was in the Western region a pronounced seasonal variation in e.g. 137 Cs content of milk. The results indicate a deficiency in scholastic achievement in the West cohort corresponding to the coincidence of the most sensitive fetal period (8-15 weeks post conception) with the 1964 late summer increase in 137 Cs content of milk. The dose from fallout is several orders of magnitude too low to explain the observed deficiency quantitatively in consonance with the Hiroshima-Nagasaki findings. It is suggested that the explaination may be found be way of a repair induction lag hypothesis, related to the microdosimetric conditions at background dose rate level. (author)

  18. On-line validation of prediction model in case of nuclear fallout

    International Nuclear Information System (INIS)

    Mueck, K.; Gerzabek, M.H.; Suda, M.; Henrich, E.

    1996-01-01

    After a large-scale nuclear fallout the early prediction of the exposure of the population to be expected is of great importance to enable early decisions on countermeasures to be taken and to optimise such decisions to ensure an maximum reduction of the expected exposure if required. This includes the prediction of the contribution of each exposure pathway, in particular the ingestion path, and the contribution of important foodstuffs to this path. The prediction should be fairly precise which requires a number of data at an early stage after the accident on a nation-wide scale. This is impeded by a number of limitations in availability of data in the early phase which are caused by various reasons: Some important data such as the activity concentration integral in air, total wet and dry deposition and radionuclide concentrations in important fodder are not available before the end of the passage of the plume and the resulting fallout. But also the time delay in taking samples of relevant items on a nation-wide scale, delivery of the samples to the measuring laboratories and the need of sample preparation especially with regard to certain non-gamma-emitting radionuclides contribute to this unavailability of data relevant for the prediction in the early phase. (author)

  19. New methodology for Ozone Depletion Potentials of short-lived compounds: n-Propyl bromide as an example

    Science.gov (United States)

    Wuebbles, Donald J.; Patten, Kenneth O.; Johnson, Matthew T.; Kotamarthi, Rao

    2001-07-01

    A number of the compounds proposed as replacements for substances controlled under the Montreal Protocol have extremely short atmospheric lifetimes, on the order of days to a few months. An important example is n-propyl bromide (also referred to as 1-bromopropane, CH2BrCH2CH3 or simplified as 1-C3H7Br or nPB). This compound, useful as a solvent, has an atmospheric lifetime of less than 20 days due to its reaction with hydroxyl. Because nPB contains bromine, any amount reaching the stratosphere has the potential to affect concentrations of stratospheric ozone. The definition of Ozone Depletion Potentials (ODP) needs to be modified for such short-lived compounds to account for the location and timing of emissions. It is not adequate to treat these chemicals as if they were uniformly emitted at all latitudes and longitudes as normally done for longer-lived gases. Thus, for short-lived compounds, policymakers will need a table of ODP values instead of the single value generally provided in past studies. This study uses the MOZART2 three-dimensional chemical-transport model in combination with studies with our less computationally expensive two-dimensional model to examine potential effects of nPB on stratospheric ozone. Multiple facets of this study examine key questions regarding the amount of bromine reaching the stratosphere following emission of nPB. Our most significant findings from this study for the purposes of short-lived replacement compound ozone effects are summarized as follows. The degradation of nPB produces a significant quantity of bromoacetone which increases the amount of bromine transported to the stratosphere due to nPB. However, much of that effect is not due to bromoacetone itself, but instead to inorganic bromine which is produced from tropospheric oxidation of nPB, bromoacetone, and other degradation products and is transported above the dry and wet deposition processes of the model. The MOZART2 nPB results indicate a minimal correction of the

  20. Radionuclide scanning

    International Nuclear Information System (INIS)

    Shapiro, B.

    1986-01-01

    Radionuclide scanning is the production of images of normal and diseased tissues and organs by means of the gamma-ray emissions from radiopharmaceutical agents having specific distributions in the body. The gamma rays are detected at the body surface by a variety of instruments that convert the invisible rays into visible patterns representing the distribution of the radionuclide in the body. The patterns, or images, obtained can be interpreted to provide or to aid diagnoses, to follow the course of disease, and to monitor the management of various illnesses. Scanning is a sensitive technique, but its specificity may be low when interpreted alone. To be used most successfully, radionuclide scanning must be interpreted in conjunction with other techniques, such as bone radiographs with bone scans, chest radiographs with lung scans, and ultrasonic studies with thyroid scans. Interpretation is also enhanced by providing pertinent clinical information because the distribution of radiopharmaceutical agents can be altered by drugs and by various procedures besides physiologic and pathologic conditions. Discussion of the patient with the radionuclide scanning specialist prior to the study and review of the results with that specialist after the study are beneficial

  1. The soil-to-plant transfer of radionuclides. Feasibilities and limits of the transfer concept

    International Nuclear Information System (INIS)

    Gerzabek, M.H.

    1993-01-01

    The present paper discusses the simple transfer model. After the Chernobyl fallout in Austria field investigations dealt with the behaviour of radionuclides in the soil-plant system. They led to the following conclusions: (1) A single plowing does not result in a homogeneous radionuclide distribution in the A p horizon. (2) Low plant availability of radionuclides (e.g. 137 Cs) led to a higher contribution of outer contamination (resuspension) to concentrations in plants in the first years after the fallout. Differences arose between high and low contamination areas. This was not true for 90 Sr, which exhibited three to ten times higher transfer factors as compared to 137 Cs. (3) The contamination source has a distinct impact on the plant availability of radionuclides. (4) In semi-natural environments radiocaesium can be bound to the biomass to a great extent, which results in significantly higher biological half-lives as compared to agricultural ecosystems. (author)

  2. Measurement of strontium 90 in the rain fall-out

    International Nuclear Information System (INIS)

    Suratman; Soedyartomo; Suhartono.

    1976-01-01

    The procedure of radioactivity measurement of strontium 90 in the rain fallout as well as the measurement of the fallout gross beta activity have been studied. In the preliminary study strontium 90 is separated from other cations especially fission products by fuming nitric acid, and radioactivity measurement is carried out in the form of strontium oxalate. Data of radioactivity measurement of strontium 90 and the gross beta activity in the fallout are given. (author)

  3. Prompt gamma activation analysis (PGAA) and short-lived neutron activation analysis (NAA) applied to the characterization of legacy materials

    International Nuclear Information System (INIS)

    English, G.A.; Firestone, R.B.; Perry, D.L.; Reijonen, J.P.; Ka-Ngo Leung; Garabedian, G.F.; Molnar, G.L.; Revay, Zs.

    2008-01-01

    Without quality historical records that provide the composition of legacy materials, the elemental and/or chemical characterization of such materials requires a manual analytical strategy that may expose the analyst to unknown toxicological hazards. In addition, much of the existing legacy inventory also incorporates radioactivity, and, although radiological composition may be determined by various nuclear-analytical methods, most importantly, gamma-spectroscopy, current methods of chemical characterization still require direct sample manipulation, thereby presenting special problems with broad implications for both the analyst and the environment. Alternately, prompt gamma activation analysis (PGAA) provides a 'single-shot' in-situ, non-destructive method that provides a complete assay of all major entrained elemental constituents. Additionally, neutron activation analysis (NAA) using short-lived activation products complements PGAA and is especially useful when NAA activation surpasses the PGAA in elemental sensitivity. (author)

  4. Precision mass measurements of very short-lived, neutron-rich Na isotopes using a radiofrequency spectrometer

    CERN Document Server

    Lunney, M D; Doubre, H; Henry, S; Monsanglant, C; De Saint-Simon, M; Thibault, C; Toader, C F; Borcea, C; Bollen, G

    2001-01-01

    Mass measurements of high precision have been performed on sodium isotopes out to $^{30}$Na using a new technique of radiofrequency excitation of ion trajectories in a homogeneous magnetic field. This method, especially suited to very short-lived nuclides, has allowed us to significantly reduce the uncertainty in mass of the most exotic Na isotopes: a relative error of 5x10$^{-7}$ was achieved for $^{28}$Na having a half-life of only 30.5 ms and 9x10$^{-7}$ for the weakly produced $^{30}$Na. Verifying and minimizing binding energy uncertainties in this region of the nuclear chart is important for clarification of a long standing problem concerning the strength of the $N$=20 magic shell closure. These results are the fruit of the commissioning of the new experimental program Mistral.

  5. Prompt gamma activation analysis (PGAA) and short-lived neutron activation analysis (NAA) applied to the characterization of legacy materials

    International Nuclear Information System (INIS)

    Firestone, Richard B; English, G.A.; Firestone, R.B.; Perry, D.L.; Reijonen, J.P.; Leung, Ka-Ngo; Garabedian, G.F.; Molnar, G.L.; Revay, Zs.

    2008-01-01

    Without quality historical records that provide the composition of legacy materials, the elemental and/or chemical characterization of such materials requires a manual analytical strategy that may expose the analyst to unknown toxicological hazards. In addition, much of the existing legacy inventory also incorporates radioactivity, and, although radiological composition may be determined by various nuclear-analytical methods, most importantly, gamma-spectroscopy, current methods of chemical characterization still require direct sample manipulation, thereby presenting special problems with broad implications for both the analyst and the environment. Alternately, prompt gamma activation analysis (PGAA) provides a 'single-shot' in-situ, non-destructive method that provides a complete assay of all major entrained elemental constituents.1-3. Additionally, neutron activation analysis (NAA) using short-lived activation products complements PGAA and is especially useful when NAA activation surpasses the PGAA in elemental sensitivity

  6. First Isochronous Time-of-Flight Mass Measurements of Short-Lived Projectile Fragments in the ESR

    International Nuclear Information System (INIS)

    Stadlmann, J.; Geissel, H.; Hausmann, M.; Nolden, F.; Radon, T.; Schatz, H.; Scheidenberger, C.; Attallah, F.; Beckert, K.; Bosch, F.; Falch, M.; Franczak, B.; Franzke, B.; Kerscher, Th.; Klepper, O.; Kluge, H.J.; Kozhuharov, C.; Loebner, K.E.G.; Muenzenberg, G.; Novikov, Yu.N.; Steck, M.; Sun, Z.; Suemmerer, K.; Weick, H.; Wollnik, H.

    2000-01-01

    A new method for precise mass measurements of short-lived hot nuclei is presented. These nuclei were produced via projectile fragmentation, separated with the FRS and injected into the storage ring ESR being operated in the isochronous mode. The revolution time of the ions is measured with a time-of-flight detector sensitive to single particles. This new method allows access to exotic nuclei with half-lives in the microsecond region. First results from this novel method obtained with measurements on neutron-deficient fragments of a chromium primary beam with half-lives down to 50 ms are reported. A precision of deltam/m ≤ 5 · 10 -6 has been achieved

  7. A phase-imaging ion-cyclotron-resonance technique for mass measurements of short-lived nuclides

    Energy Technology Data Exchange (ETDEWEB)

    Eliseev, Sergey; Blaum, Klaus; Doerr, Andreas; Eronen, Tommi; Goncharov, Mikhail; Hoecker, Martin; Ketter, Jochen; Ramirez, Enrique Minaya; Simon, Vanessa [Max-Planck Institute for Nuclear Physics (Germany); Block, Michael [GSI Helmholtzzentrum fuer Schwerionenforschung GmbH (Germany); Chenmarev, Stanislav; Filjanin, Pavel; Nesterenko, Dmitriy; Novikov, Yuri [Petersburg Nuclear Physics Institute (Russian Federation); Droese, Christian; Schweikhard, Lutz [Institute for Physics, Ernst-Moritz-Arndt-University (Germany)

    2014-07-01

    A novel approach to mass measurements on the sub-ppb level even for short-lived nuclides with half-lives well below one second is presented. It is based on the projection of the radial ion motion in a Penning trap onto a position sensitive detector. Compared to the presently employed time-of-flight ion-cyclotron-resonance technique, the novel approach is 25-times faster and provides a 40-fold gain in resolving power. With the new technique low-lying isomeric states with excitation energy on the 10-keV level can be separated from the ground state. Moreover, the new technique possesses a substantially higher sensitivity since just two ions are sufficient to determine the ion cyclotron frequency. A measurement of the mass difference of singly charged ions of {sup 132}Xe and {sup 131}Xe with an uncertainty of 25 eV has demonstrated the great potential of the new approach.

  8. Release studies of a thin foil tantalum target for the production of short-lived radioactive nuclei

    CERN Document Server

    Bennett, J R J; Drumm, P V; Lettry, Jacques; Nilsson, T; Catherall, R; Jonsson, O C; Ravn, H L; Simon, H

    2002-01-01

    Measurements have been made at ISOLDE, of the release curves and yields of radioactive beams of lithium, sodium and beryllium from a target constructed from 2 $\\mu$m thick foils. The release curves have been analysed by fitting to a mathematical model to determine the coefficients of diffusion of the particles in the foils and effusion through the target and ionizer at several temperatures. Through a better understanding of the rate of transport of the particles, it is possible to design targets and ionizers with improved yields. This is most important for the rare, short-lived isotopes in which there is considerable interest for physics experiments. This target has demonstrated large increases in the yields of $^{11}$Li and $^{12}$Be, in agreement with the predictions of the model. (11 refs).

  9. Transuranic radionuclides dispersed into the aquatic environment, a bibliography

    Energy Technology Data Exchange (ETDEWEB)

    Noshkin, V.E.; Stoker, A.C.; Wong, Kai M. [and others

    1994-04-01

    The purpose of this project was to compile a bibliography of references containing environmental transuranic radionuclide data. Our intent was to identify those parameters affecting transuranic radionuclide transport that may be generic and those that may be dependent on chemical form and/or environmental conditions (i.e., site specific) in terrestrial, aquatic and atmospheric environments An understanding of the unique characteristics and similarities between source terms and environmental conditions relative to transuranic radionuclide transport and cycling will provide the ability to assess and predict the long term impact on man and the environment. An additional goal of our literature review, was to extract the ranges of environmental transuranic radionuclide data from the identified references for inclusion in a data base. Related to source term, these ranges of data can be used to calculate the dose to man from the radionuclides, and to perform uncertainty analyses on these dose assessments. On the basis of our reviews, we have arbitrarily outlined five general source terms. These are fallout, fuel cycle waste, accidents, disposal sites and resuspension. Resuspension of the transuranic radionuclides is a unique source term, in that the radionuclides can originate from any of the other source terms. If these transuranic radionuclides become resuspended into the air, they then become important as a source of inhaled radionuclides.

  10. Analysis of the performance and usefulness of a new digital gamma camera and short-lived radionuclide Au-195m for cardiac studies

    International Nuclear Information System (INIS)

    Mena, I.; Amaral, H.; Adams, R.; Garcia, E.; de Jong, R.

    1983-01-01

    The purpose of this investigation is to evaluate at LAC Harbor-UCLA Medical Center dead time characteristics of the digital camera Elscint (Apex 415), designed by the manufacturer to improve the count rate performance, its resolution and clinical applications in first pass ventriculography. The Hg-195m/Au-195m generator is evaluated for Hg-195 leakage, dosimetry and clinical usefulness. The high count rate capability of the digital camera is maximally utilized in biplane ventriculography which may become the optimal modality for dynamic cardiovascular nuclear medicine studies. The resolution achieved in this high count rate modality appears perfectly adequate for high quality studies. The imaging and radiation exposure characteristics of the 30.5 sec half life Au 195m are promising of a significant clinical contribution in the field of adult and pediatric cardiology

  11. Thyroid cancer in the Marshallese: relative risk of short-lived internal emitters and external radiation exposure

    International Nuclear Information System (INIS)

    Lessard, E.T.; Brill, A.B.; Adams, W.H.

    1985-01-01

    In a study of the comparative effects of internal versus external irradiation of the thyroid in young people, we determined that the dose from internal irradiation of the thyroid with short-lived internal emitters produced several times less thyroid cancer than did the same dose of radiation given externally. We determined this finding for a group of 85 Marshall Islands children, who were less than 10 years of age at the time of exposure and who were accidentially exposed to internal and external thyroid radiation at an average level of 1400 rad. The external risk coefficient ranged between 2.5 and 4.9 cancers per million person-rad-years at risk, and thus, from our computations, the internal risk coefficient for the Marshallese children was estimated to range between 1.0 and 1.4 cancers per million person-rad-years at risk. In contrast, for individual more than 10 years of age at the time of exposure, the dose from internal irradiation of the thyroid with short-lived internal emitters produced several times more thyroid cancer than did the same dose of radiation given externally. The external risk coefficients for the older age groups were reported in the literature to be in the range of 1.0 to 3.3 cancers per million person-rad-years-at risk. We computed internal risk coefficients of 3.3 to 8.1 cancers per million person-rad-years at risk for adolescent and adult groups. This higher sensitivity to cancer induction in the exposed adolescents and adults, is different from that seen in other exposed groups. 14 refs., 8 tabs

  12. Thyroid cancer in the Marshallese: relative risk of short-lived internal emitters and external radiation exposure

    International Nuclear Information System (INIS)

    Lessard, E.T.; Brill, A.B.; Adams, W.H.

    1986-01-01

    In a study of the comparative effects of internal versus external irradiation of the thyroid in young people, we determined that the dose from internal irradiation of the thyroid with short-lived internal emitters produced several times less thyroid cancer than did the same dose of radiation given externally. The authors determined this finding for a group of 85 Marshall Islands children, who were less than 10 years of age at the time of exposure and who were accidentally exposed to internal and external thyroid radiation at an average level of 1400 rad. The external risk coefficient ranged between 2.5 and 4.9 cancers per million person-rad-years at risk, and thus, from our computations, the internal risk coefficient for the Marshallese children was estimated to range between 1.0 and 1.4 cancers per million person-rad-years at risk. In contrast, for individuals more than 10 years of age at the time of exposure, the dose from internal irradiation of the thyroid with short-lived internal emitters produced several times more thyroid cancer than did the same dose of radiation given externally. The external risk coefficients for the older age groups were reported in the above literature to be in the range of 1.0 to 3.3 cancers per million person-rad-years-at risk. The authors computed internal risk coefficients of 3.3 to 8.1 cancers per million person-rad-years at risk for adolescent and adult groups. This higher sensitivity to cancer induction in the exposed adolescents and adults, is different from that seen in other exposed groups. The small number of cancers in the exposed population and the influence of increased levels of TSH, nonuniform irradiation of the thyroid, and thyroid cell killing at high dose make it difficult to draw firm conclusions from these studies. 14 references, 8 tables

  13. Radioactive fallout collected in Tokyo on November 26, 1955

    Energy Technology Data Exchange (ETDEWEB)

    Sugiura, Y; Kanazawa, T

    1956-01-01

    A large nuclear weapon test by Russia was reported November 23, 1955 as having occurred the previous day. Rain water and fallout samples taken in Tokyo before and after the 22nd indicated the test had produced a secondary fallout from some previous explosion. Rain water of the 21st and fallout of the 29th had radioactive content of 13 days half-life; fallout of the 26th, rain of the 27th 3 days half-life. Sample of the 26th consisted of 15 mg of sooty material giving nearly 2000 counts/min at that time.

  14. Accumulation of radionuclides by lichen symbionts

    Energy Technology Data Exchange (ETDEWEB)

    Nifontova, M G; Kulikov, N V [AN SSSR, Sverdlovsk. Inst. Ehkologii Rastenij i Zhivotnykh

    1983-01-01

    The aim of investigation is the quantitative estimation of ability and role of separate symbionts in the accumulation of radionuclides. As investigation volumes, durably cultivated green lichen alga Trebouxia erici and lichen fungi extracted from Cladonia rangiferina, Parmelia caperata and Acarospora fuscata are used. The accumulation of radioactive isotopes with fungi and seaweeds is estimated according to accumulation coefficients (AC) which are the ratio of radiation concentration in plants and agarized medium. Radionuclide content (/sup 90/Sr and /sup 137/Cs) is determined radiometrically. A special series of experiments is done to investigate radionuclide accumulation dependences with lichen seaweed and fungi on light conditions. It is shown that both symbionts of lichen-seaweed and fungus take part in the accumulation of radionuclide from outer medium (atmospheric fall-out and soil). However fungus component constituting the base of structural organization of thallus provides the greater part of radionuclides accumulated by the plant. Along with this the violation of viability of seaweed symbionts particularly in the case of light deficiency brings about the reduction of /sup 137/Cs sorption by seaweeds and tells on the total content of radiocesium in plant thallus.

  15. Balance of anthropogenic radionuclides in the Japan Sea

    International Nuclear Information System (INIS)

    Tsuneyama, Teppei; Ito, Toshimichi; Otosaka, Shigeyoshi

    2007-01-01

    Concentration data of 90 Sr, 137 Cs and 239+240 Pu between 1960 and 2002 were examined to estimate the balance of anthropogenic radionuclides in water of the Japan Sea. Until 1960s, they had accumulated mainly in the upper layer of the Japan Sea. After that, the amount of the radionuclides decreased as a result of termination of global fallout and exchange of surface water. The trend turned into increase since 1980s and the amounts will continue to increase for a while. (author)

  16. Radioactive fallout has different effects in Lapland

    International Nuclear Information System (INIS)

    Rissanen, K.

    1993-01-01

    The effects of radioactive fallout in Lapland differ from those in southern Finland. The subarctic area is poor in vegetation and nutrients, for which reason radioactive substances enter food chains rapidly. As potassium is low in supply in the north, plants use cesium to replace it. Thus cesium is accumulated very effectively in food chain. When in the food chain, cesium is enriched in reindeer and further in Lapp people, who eat reindeer meat frequently. The Finnish Centre for Radiation and Nuclear Safety established a regional laboratory in northern Finland in the 1970's to monitor radiation and carry out research an the area.(author)

  17. Fallout: The experiences of a medical team in the care of a Marshallese population accidently exposed to fallout radiation

    International Nuclear Information System (INIS)

    Conard, R.A.

    1992-09-01

    This report presents an historical account of the experiences of the Brookhaven Medical Team in the examination and treatment of the Marshallese people following their accidental exposure to radioactive fallout in 1954. This is the first time that a population has been heavily exposed to radioactive fallout, and even though this was a tragic mishap, the medical findings have provided valuable information for other accidents involving fallout such as the recent reactor accident at Chernobyl. Noteworthy has been the unexpected importance of radioactive iodine in the fallout in producing thyroid abnormalities

  18. Fallout: The experiences of a medical team in the care of a Marshallese population accidentally exposed to fallout radiation

    International Nuclear Information System (INIS)

    Conard, R.A.

    1991-01-01

    This report presents an historical account of the experiences of the Brookhaven Medical team in the examination and treatment of the Marshallese people following their accidental exposure to radioactive fallout in 1954. This is the first time that a population has been heavily exposed to radioactive fallout, and even though this was a tragic mishap, the medical findings have provided valuable information for other accidents involving fallout such as the recent reactor accident at Chernobyl. Particularly important has been the unexpected importance of radioactive iodine in the fallout in producing thyroid abnormalities

  19. Fallout: The experiences of a medical team in the care of a Marshallese population accidentally exposed to fallout radiation

    Energy Technology Data Exchange (ETDEWEB)

    Conard, R.A.

    1991-12-31

    This report presents an historical account of the experiences of the Brookhaven Medical team in the examination and treatment of the Marshallese people following their accidental exposure to radioactive fallout in 1954. This is the first time that a population has been heavily exposed to radioactive fallout, and even though this was a tragic mishap, the medical findings have provided valuable information for other accidents involving fallout such as the recent reactor accident at Chernobyl. Particularly important has been the unexpected importance of radioactive iodine in the fallout in producing thyroid abnormalities.

  20. Fallout: The experiences of a medical team in the care of a Marshallese population accidentally exposed to fallout radiation

    Energy Technology Data Exchange (ETDEWEB)

    Conard, R.A.

    1991-01-01

    This report presents an historical account of the experiences of the Brookhaven Medical team in the examination and treatment of the Marshallese people following their accidental exposure to radioactive fallout in 1954. This is the first time that a population has been heavily exposed to radioactive fallout, and even though this was a tragic mishap, the medical findings have provided valuable information for other accidents involving fallout such as the recent reactor accident at Chernobyl. Particularly important has been the unexpected importance of radioactive iodine in the fallout in producing thyroid abnormalities.

  1. Fallout: The experiences of a medical team in the care of a Marshallese population accidently exposed to fallout radiation

    Energy Technology Data Exchange (ETDEWEB)

    Conard, R.A.

    1992-09-01

    This report presents an historical account of the experiences of the Brookhaven Medical Team in the examination and treatment of the Marshallese people following their accidental exposure to radioactive fallout in 1954. This is the first time that a population has been heavily exposed to radioactive fallout, and even though this was a tragic mishap, the medical findings have provided valuable information for other accidents involving fallout such as the recent reactor accident at Chernobyl. Noteworthy has been the unexpected importance of radioactive iodine in the fallout in producing thyroid abnormalities.

  2. Radionuclide migration in the Chernobyl contamination zone

    International Nuclear Information System (INIS)

    Golosov, V.N.; Panin, A.V.; Ivanova, N.N.

    1998-01-01

    It is well known that fallout of 137 Cs reaching the land soils with precipitation was rapidly and tightly sorbed to the fine fraction of sediment or soils. The majority of the 137 Cs is retained in the top few centimetres of the soil or sediment profiles (Loughran et al, 1993, Owens et al, 1996). In the absence of strong variations in precipitation over a relatively small area the total bomb-derived 137 Cs fallout can assumed to be spatial uniform. The Chernobyl 137 Cs fallout was mostly connected with one or two rains. So the spatial variability of this 137 Cs can be higher. Furthermore because the explosion on the Chernobyl nuclear plant happen together with fire, a lot of ashes particles with radionuclide were distributed within vast areas. So even microvariability of Chernobyl 137 Cs can be very high in some places. The horizontal migration of 137 Cs connects with soil erosion processes that dominate on the agricultural lands of the Central Russia. The main goal of this investigation is to evaluate the caesium-137 horizontal and vertical migration within typical landscape of the Central Russia 11 years after the Chernobyl accident

  3. Measurements of Background and Fall-out T Radioactivity in Samples from the Baltic Bay of Tvaeren, 1957-1963

    Energy Technology Data Exchange (ETDEWEB)

    Agnedahl, P O

    1965-01-15

    To get information on the possible effects of future releases of radioactive effluents into Tvaeren, a bay of the Baltic, the Atomic Energy Company has had to carry out a biological and radiological programme in Tvaeren. The work was scheduled to extend over at least two years but in fact proceeded from 1957 to 1963. Unfortunately, no exact idea of the natural activity could be gained on account of the fallout from the repeated atomic bomb tests. Instead, the work developed into a study of the variations in biological samples caused by these tests. This report studies the correlation between the activity in fallout and that in flora and fauna. The contribution of natural activity from the radionuclide K-40 has been determined and is given for all samples. The following values may be regarded as representative of total {beta}-activity and activity of K-40 in the investigated samples. T 1204 has been used as standard.

  4. Radionuclide examinations

    International Nuclear Information System (INIS)

    Lentle, B.C.

    1989-01-01

    This paper reports on radionuclide examinations of the pancreas. The pancreas, situated retroperitonally high in the epigastrium, was a particularly difficult organ to image noninvasively before ultrasonography and computed tomography (CT) became available. Indeed the organ still remains difficult to examine in some patients, a fact reflected in the variety of methods available to evaluate pancreatic morphology. It is something of a paradox that the pancreas is metabolically active and physiologically important but that its examination by radionuclide methods has virtually ceased to have any role in day-to-day clinical practice. To some extent this is caused by the tendency of the pancreas's commonest gross diseases emdash carcinoma and pancreatitis, for example emdash to result in nonfunction of the entire organ. Disorders of pancreatic endocrine function have generally not required imaging methods for diagnosis, although an understanding of diabetes mellitus and its nosology has been advanced by radioimmunoassay of plasma insulin concentrations

  5. Field surveying of radionuclide contamination in forests

    International Nuclear Information System (INIS)

    Turunen, J.; Rantavaara, A.; Ammann, M.

    2009-01-01

    Field measurements of radionuclides after an accidental contamination of forests assume the capacity for identification of a number of nuclides in varying source geometries. The continuous redistribution of radionuclides in forests through natural processes implies a decrease of prevailing surface contamination of trees and an increase in activity density on the ground. Portable gamma spectrometers have long been based on Na(I) detectors which, due to their low energy resolution, are not the tool for analysis of contamination from accidental releases of fission and activation products in the first days or weeks after a deposition. Data of airborne radionuclides from the Chernobyl accident in April 1986 were used for demonstration of initial and later distribution of radionuclides as sources of air Kerma in forests. Forest model (FDMF, PV. 6.0) of the RODOS system was used for the assessment of time-dependent Kerma rate from different forest compartments. The results show the fast reduction of activities of short-lived nuclides and their contributions to the Kerma rate in the first weeks and months. The results also give an estimate for the time needed until a gamma spectrometer with a low energy resolution would give useful information about long-lived radioactivity on the forest floor. An example is given on a portable high resolution semiconductor spectrometer that has suitable characteristics for field surveying also during occurrence of a great number of radionuclides contributing to the gamma spectrum. The needs for further research of a recently deposited radionuclide contamination on forest vegetation and soil, and the efforts for improvement of portable radiation meters and their use in management planning and radioecological research on contaminated forests are discussed. (au)

  6. Production of selected cosmogenic radionuclides by muons; 1, Fast muons

    CERN Document Server

    Heisinger, B; Jull, A J T; Kubik, P W; Ivy-Ochs, S; Neumaier, S; Knie, K; Lazarev, V A; Nolte, E

    2002-01-01

    To investigate muon-induced nuclear reactions leading to the production of radionuclides, targets made of C/sub 9/H/sub 12/, SiO /sub 2/, Al/sub 2/O/sub 3/, Al, S, CaCO/sub 3/, Fe, Ni, Cu, Gd, Yb and Tl were irradiated with 100 and 190 GeV muons in the NA54 experimental setup at CERN. The radionuclide concentrations were measured with accelerator mass spectrometry and gamma -spectroscopy. Results are presented for the corresponding partial formation cross- sections. Several of the long-lived and short-lived radionuclides studied are also produced by fast cosmic ray muons in the atmosphere and at depths underground. Because of their importance to Earth sciences investigations, calculations of the depth dependence of production rates by fast cosmic ray muons have been made. (48 refs).

  7. Radionuclide transfer

    International Nuclear Information System (INIS)

    Gerber, G.B.

    1993-01-01

    The research project described here had the aim to obtain further information on the transfer of nuclides during pregnancy and lactation. The tests were carried out in mini-pigs and rats receiving unchanging doses of radionuclides with the food. The following findings were revealed for the elements examined: Fe, Se, Cs and Zn were characterized by very high transfer levels in the mother, infant and foetus. A substantial uptake by the mother alone was observed for Co, Ag and Mn. The uptake by the foetus and infant here was 1 to 10 times lower. A preferential concentration in certain tissues was seen for Sr and Tc; the thyroid levels of Tc were about equally high in mothers and infants, while Sr showed less accumulation in the maternal bone. The lanthanide group of substances (Ce, Eu and Gd as well as Y and Ru) were only taken up to a very limited extent. The uptake of the examined radionuclides (Fe, Co, Ag, Ce) with the food ingested was found here to be ten times greater in rats as compared to mini-pigs. This showed that great caution must be observed, if the behaviour of radionuclides in man is extrapolated from relevant data obtained in rodents. (orig./MG) [de

  8. Use of standard spectra for the short life radionuclides and ratios for long life radionuclides in the wastes of EDF PWR type reactors

    International Nuclear Information System (INIS)

    Lantes, B.; Bienvenu, Ph.

    2001-01-01

    This paper presents the type of declaration of radioactivity in the wastes of PWR type reactors park. Particularly, it insists on the justification of use of spectra for the declaration of short live radionuclides. It tackles the important developments of methods and measures of radiochemical analysis made by the Cea in order to determine the ratios to declare the long life radioisotopes. (N.C.)

  9. Fallout and drinking water contamination by I-131 and Cs-134, 137 in Japan, from the Fukushima Daiichi NPS accident

    International Nuclear Information System (INIS)

    Kelecom, Alphonse; Miyashita, Erika; Kelecom, Patrick Vicent

    2011-01-01

    The earthquake followed by a tsunami in Japan, on last March 11, seriously damaged four of the six reactors of the Fukushima Daiichi nuclear power station (NPS). Radioactive smokes and highly contaminated water were released for weeks to the environment. Since March 12, when the plant operator TEPCO and Japan's nuclear agency (NISA) confirmed the presence of radionuclides near the NPS, a giant environmental monitoring operation was set up, covering the entire Japanese territory. Daily thousands measurements are realized. We here analyze data released during 60 days on I-131 and Cs-134,137 radioactive concentrations in drinking water and fallout for 45 prefectures. Miyagi and Fukushima, that requires a separate study, are not considered here. Drinking water contamination by I-131 was observed in 13 prefectures, including Tokyo. The most impacted one was Tochigi (maximum of 110 Bq/l, March 24). This value turned water not drinkable for infants and babies. Cs-137 was detected in drinking water in 8 prefectures, with a maximum level of 18 Bq/l in Ibaraki. These levels do not affect potability of tap water. I-131 was observed in fallout in 27 prefectures, with level reaching 93 kBq/m2 in Ibaraki and 36 kBq/m 2 in Tokyo on March 21 and 23 respectively. Fallout of Cs-137 was observed in 19 prefectures. The maximum deposition occurred again in Ibaraki (13kBq/m 2 , March 21) and in Tokyo (5.3 kBq/m2, March 22). Since mid April, only trace contamination has been observed for both radionuclides in drinking water. Sporadically medium levels of Cs-137 are still observed in fallout. (author)

  10. Fallout and drinking water contamination by I-131 and Cs-134, 137 in Japan, from the Fukushima Daiichi NPS accident

    Energy Technology Data Exchange (ETDEWEB)

    Kelecom, Alphonse; Miyashita, Erika; Kelecom, Patrick Vicent [Universidade Federal Fluminense (UFF), Niteroi, RJ (Brazil)

    2011-07-01

    The earthquake followed by a tsunami in Japan, on last March 11, seriously damaged four of the six reactors of the Fukushima Daiichi nuclear power station (NPS). Radioactive smokes and highly contaminated water were released for weeks to the environment. Since March 12, when the plant operator TEPCO and Japan's nuclear agency (NISA) confirmed the presence of radionuclides near the NPS, a giant environmental monitoring operation was set up, covering the entire Japanese territory. Daily thousands measurements are realized. We here analyze data released during 60 days on I-131 and Cs-134,137 radioactive concentrations in drinking water and fallout for 45 prefectures. Miyagi and Fukushima, that requires a separate study, are not considered here. Drinking water contamination by I-131 was observed in 13 prefectures, including Tokyo. The most impacted one was Tochigi (maximum of 110 Bq/l, March 24). This value turned water not drinkable for infants and babies. Cs-137 was detected in drinking water in 8 prefectures, with a maximum level of 18 Bq/l in Ibaraki. These levels do not affect potability of tap water. I-131 was observed in fallout in 27 prefectures, with level reaching 93 kBq/m2 in Ibaraki and 36 kBq/m{sup 2} in Tokyo on March 21 and 23 respectively. Fallout of Cs-137 was observed in 19 prefectures. The maximum deposition occurred again in Ibaraki (13kBq/m{sup 2}, March 21) and in Tokyo (5.3 kBq/m2, March 22). Since mid April, only trace contamination has been observed for both radionuclides in drinking water. Sporadically medium levels of Cs-137 are still observed in fallout. (author)

  11. 182Hf-182W age dating of a 26Al-poor inclusion and implications for the origin of short-lived radioisotopes in the early Solar System

    DEFF Research Database (Denmark)

    Holst, Jesper Christian; Olsen, Mia Bjørg Stolberg; Paton, Chad

    2013-01-01

    provide a unique window into the earliest Solar System, including the origin of short-lived radioisotopes. However, their chronology is unknown. Using the 182Hf–182W chronometer, we show that a FUN CAI recording a condensation origin from a solar gas formed coevally with canonical CAIs, but with 26Al/27Al......Refractory inclusions [calcium–aluminum-rich inclusions, (CAIs)] represent the oldest Solar System solids and provide information regarding the formation of the Sun and its protoplanetary disk. CAIs contain evidence of now extinct short-lived radioisotopes (e.g., 26Al, 41Ca, and 182Hf) synthesized...... in one or multiple stars and added to the protosolar molecular cloud before or during its collapse. Understanding how and when short-lived radioisotopes were added to the Solar System is necessary to assess their validity as chronometers and constrain the birthplace of the Sun. Whereas most CAIs formed...

  12. Radioactive fallout and neural tube defects | Akar | Egyptian Journal ...

    African Journals Online (AJOL)

    Possible link between radioactivity and the occurrence of neural tube defects is a long lasting debate since the Chernobyl nuclear fallout in 1986. A recent report on the incidence of neural defects in the west coast of USA, following Fukushima disaster, brought another evidence for effect of radioactive fallout on the ...

  13. The isotopic signature of fallout plutonium in the North Pacific

    International Nuclear Information System (INIS)

    Buesseler, K.O.

    1997-01-01

    Plutonium analyses of a dated coral record from the French Frigate Shoals in the central North Pacific indicate that there are two major sources of Pu in this basin: close-in (tropospheric) fallout from nuclear weapons testing at the Pacific Proving Grounds in the Marshall Islands in the 1950s and global (stratospheric) fallout which peaked in 1962. Furthermore, the 240 Pu/ 239 Pu atom ratio of fallout from the Pacific Proving Grounds is characteristically higher (0.24) than that of global fallout Pu (0.18-0.19). Seawater and sediment samples from the North Pacific exhibit a wide range of 240 Pu/ 239 Pu values (0.19-0.34), with a trend towards higher ratios in the subsurface waters and sediment. Deep water 240 Pu/ 239 Pu ratios are higher in the vicinity of the Marshall Islands relative to stations further from this close-in fallout source. These preliminary data suggest that fallout Pu from the Pacific Proving Grounds is more rapidly removed from the surface waters than is global fallout Pu. Plutonium geochemistry appears to be related to the physical/chemical form of Pu-bearing particles generated by different fallout sources. (author)

  14. The isotopic signature of fallout plutonium in the North Pacific

    Energy Technology Data Exchange (ETDEWEB)

    Buesseler, K.O. [Woods Hole Oceanographic Institution, MA (United States)

    1997-07-01

    Plutonium analyses of a dated coral record from the French Frigate Shoals in the central North Pacific indicate that there are two major sources of Pu in this basin: close-in (tropospheric) fallout from nuclear weapons testing at the Pacific Proving Grounds in the Marshall Islands in the 1950s and global (stratospheric) fallout which peaked in 1962. Furthermore, the {sup 240}Pu/{sup 239}Pu atom ratio of fallout from the Pacific Proving Grounds is characteristically higher (0.24) than that of global fallout Pu (0.18-0.19). Seawater and sediment samples from the North Pacific exhibit a wide range of {sup 240}Pu/{sup 239}Pu values (0.19-0.34), with a trend towards higher ratios in the subsurface waters and sediment. Deep water {sup 240}Pu/{sup 239}Pu ratios are higher in the vicinity of the Marshall Islands relative to stations further from this close-in fallout source. These preliminary data suggest that fallout Pu from the Pacific Proving Grounds is more rapidly removed from the surface waters than is global fallout Pu. Plutonium geochemistry appears to be related to the physical/chemical form of Pu-bearing particles generated by different fallout sources. (author).

  15. Status of radionuclide monitoring stations in Australia

    International Nuclear Information System (INIS)

    Burns, P.A.

    2001-01-01

    The Australian Radiation Protection and Nuclear Safety Agency (ANSTO) first became involved in the monitoring of radionuclides in the environment in 1955 when assessing the effects on the Australian population of the radioactive releases associated with the atmospheric testing of nuclear weapons. (At that time ARPANSA was known as the Commonwealth X-ray and Radium Laboratory). The United Kingdom had tested weapons in Australia in 1952 and 1953 and in August 1954 entered into an agreement with the Australian Government to establish a test range at Maralinga in South Australia. The government established a Maralinga Safety Committee and through this Committee ARPANSA became involved in the surveillance of radioactive fallout over Australia. The primary function of this surveillance was to ensure that the nuclear trials would not adversely effect the health of the Australian population. A program was established to reliably assess the deposition of radioactive fallout over Australia so that exposure to the population could be estimated. This task was performed in conjunction with the Bureau of Meteorology and the Department of Supply. Measurements were made on daily samples of fallout dawn from 10 centres throughout Australia. A low level radiochemical facility was established in 1961 for the measurement of 90 Sr and 137 Cs in environmental samples so that the long term distribution of fallout could be tracked. In the 1960s the program was extended to measure fresh fission products reaching Australia from atmospheric testing in other countries, usually originating from test sites in the northern hemisphere. The sampling program that was established was designed so that it could be rapidly expanded when a new testing program started. At this time a permanent fallout monitoring network was established around Australia using high volume air samplers capable of sampling up to 10000 m 3 per week. Approximately six stations have been operated at any one time but the

  16. Dynamics and balance of natural and anthropic radionuclide particulates in the Gulf of Lion: the case of Rhone river transports

    International Nuclear Information System (INIS)

    Marion, Cedric

    2010-01-01

    The aim of this study was to evaluate and understand particulate transfers dynamics and balances of radionuclides in the Gulf of Lion, particularly at the Rhone River mouth. Due to its 30.2 year half-life and of its great affinity with silts and clays, 137 Cs was used as a Rhone River inputs tracer. Rhone pro-delta sediments recorded values of 137 Cs activities originated by nuclear power plants releases, global fallout and Chernobylsk accident (peak at 600 Bq.kg-1). A sharp decrease in liquid radioactive effluents releases and the dismantlement of the Marcoule fuel reprocessing plant in 1997 induced 137 Cs fluxes decrease to the Mediterranean Sea. At present time, mean concentrations are around 10 Bq.kg-1 in the pro-delta sediments. Sedimentary records of different oceanographic campaigns achieved between 2001 and 2008 enabled to map a 20 km 2 137 Cs accumulation area close to the Rhone River mouth and to estimate a store of 3.35 TBq, i.e. the eighth of the Gulf of Lions store, which area is about 15000 km 2 . Other campaigns carried out in the framework of the CARMA and EXTREMA projects (2006-2008) allowed to observe surface and bottom nepheloids behaviours and to link them to the pro-delta sedimentation. Radio-chronological analyses coupling 137 Cs and 210 Pb depth activity profiles allowed to estimate pluri-deci-metric accumulation rates next to the mouth. Short-live radionuclides like 7 Be and 234 Th were used to estimate sedimentary deposits thicknesses generated by some Rhone River floods. These results were confirmed by an experiment which induced an instruments deployment at the Rhone River mouth during the winter 2006-2007. Altimeter data showed 8 cm thick sediment total accretion during two mean floods recorded by a current profiler. They also showed an important erosion phase linked to a south-east swell episode with a bottom shear stress reaching 5 Pa. An erodimeter enabled to evaluate the erosion shear stress threshold to 0.35 Pa next to the mouth

  17. A survey of selected neutron-activation reactions with short-lived products of importance to fusion reactor technology

    International Nuclear Information System (INIS)

    Ward, R.C.; Gomes, I.C.; Smith, D.L.

    1994-11-01

    The status of the cross sections for production of short-lived radioactivities in the intense high-energy neutron fields associated with D-T fusion reactors is investigated. The main concerns relative to these very radioactive isotopes are with radiation damage to sensitive components such as superconducting magnets, the decay-heat problem and the safety of personnel during operation of the facility. The present report surveys the status of nuclear data required to assess these problems. The study is limited to a few high-priority nuclear reactions which appear to be of critical concern in this context. Other reactions of lesser concern are listed but are not treated in the present work. Among the factors that were considered in defining the relevant reactions and setting priorities are: quantities of the elemental materials in a fusion reactor, isotopic abundances within elemental categories, the decay properties of the induced radioactive byproducts, the reaction cross sections, and the nature of the decay radiations. Attention has been focused on radioactive species with half lives in the range from about 1 second to 15 minutes. Available cross-section and reaction-product decay information from the literature has been compiled and included in the report. Uncertainties have been estimated by examining several sets of experimental as well as evaluated data. Comments on the general status of data for various high-priority reactions are offered. On the basis of this investigation, it has been found that the nuclear data are in reasonably good shape for some of the most important reactions but are unacceptable for others. Based on this investigation, the reactions which should be given the greatest attention are: 16 O(n,p) 16 N, 55 Mn(n,p) 55 Cr, 57 Fe(n,p) 57 Mn, 186 W(n,2n) 185m W, and 207 Pb(n,n') 207m Pb. However, the development of fusion power would benefit from an across-the-board refinement in these nuclear data so that a more accurate quantitative

  18. Hygienic estimation of population doses due to stratospheric fallout

    International Nuclear Information System (INIS)

    Marej, A.N.; Knizhnikov, V.A.

    1980-01-01

    The hygienic estimation of external and internal irradiation of the USSR population due to stratospheric global fallouts of fission products after nuclear explosions and weapon tests, is carried out. Numerical values which characterize the dose-effect dependence in the case of radiation of marrow, bone tissue and whole body are presented. Values of mean individual and population doses of irradiation due to global fallouts within 1963-1975, types of injury and the number of mortal cases due to malignant neoplasms are presented. A conclusion is made that the contribution of radiation due to stratospheric fallouts in the mortality due to malignant neoplasms is insignificant. Annual radiation doses, conditioned by global fallouts within the period of 1963-1975 constitute but several percent from the dose of radiation of the natural radiation background. Results of estimation of genetic consequences of irradiation due to atmospheric fallouts are presented

  19. Radionuclide radiology

    International Nuclear Information System (INIS)

    Scarsbrook, A.F.; Graham, R.N.J.; Perriss, R.W.; Bradley, K.M.

    2006-01-01

    This is the fourth in a series of short reviews of internet-based radiological educational resources, and will focus on radionuclide radiology and nuclear medicine. What follows is a list of carefully selected websites to save time in searching them out. Most of the sites cater for trainee or non-specialist radiologists, but may also be of interest to specialists for use in teaching. This article may be particularly useful to radiologists interested in the rapidly expanding field of positron emission tomography computed tomography (PET-CT). Hyperlinks are available in the electronic version of this article and were all active at the time of going to press (February 2006)

  20. The investigation of properties of short-lived SF isotopes (Z > 100 at the focal plane of VASSILISSA separator

    Directory of Open Access Journals (Sweden)

    Svirikhin Alexandr

    2013-12-01

    Full Text Available For experiments aimed at the study of spontaneous fission of transfermium nuclei improvements in the focal plane detector system of recoil separator VASSILISSA have been made. A neutron detector consisting of 54 3He-filled counters has been mounted around the focal-plane detector chamber. The reaction 48Ca + 206Pb = 2n + 252No is used for tuning the separator settings and calibrating the detector system with the spontaneous fission of the 252No. The average neutron number per 252No spontaneous fission event is as large as ν̅ = 4.06 ± 0.12. The short-lived heavy isotopes 244,246Fm, produced in the complete fusion reactions 40Ar + 206,208Pb, are investigated. The average number of neutrons per spontaneous fission of 244,246Fm from the experimental data were (ν̅ = 3.3 ± 0.3 and (ν̅ = 3.55 ± 0.50, respectively. Both values are determined for the first time.

  1. Neutron-captures in Low Mass Stars and the Early Solar System Record of Short-lived Radioactivities

    Science.gov (United States)

    Busso, Maurizio; Vescovi, Diego; Trippella, Oscar; Palmerini, Sara; Cristallo, Sergio; Piersanti, Luciano

    2018-01-01

    Noticeable improvements were recently introduced in the modelling of n-capture nucleosynthesis in the advanced evolutionary stages of giant stars (Asymptotic Giant Branch, or AGB, stars). Two such improvements are closely linked together and concern the introduction of non-parameterized, physical models for extended mixing processes and the adoption of accurate reaction rates for H- and He-burning reactions, including the one for the main neutron source 13C(α,n)16O. These improvements profited of a longstanding collaboration between stellar physicists and C. Spitaleri's team and of his seminal work both as a leader in the Nuclear Astrophysics scenario and as a talent-scout in the recruitment of young researchers in the field. We present an example of the innovative results that can be obtained thanks to the novelties introduced, by estimating the contributions from a nearby AGB star to the synthesis of short-lived (t1/2 ≤ 10 Myr) radioactive nuclei which were alive in early Solar System condensates. We find that the scenario indicating an AGB star as the source of such radioactivities, discussed for many years by researchers in this field, appears now to be no longer viable, when the mentioned improvements of AGB models and nuclear parameters are considered.

  2. Simulation study on the measurements of diffusion coefficients in solid materials by short-lived radiotracer beams

    CERN Document Server

    Jeong, S C; Kawakami, H

    2003-01-01

    We have examined, by a computer simulation, an on-line measurement of diffusion coefficients by using a short-lived alpha particle emitter, sup 8 Li (half life of 0.84s), as a radiotracer. The energy spectra of alpha particles emitted from diffusing sup 8 Li primarily implanted in the sample of LiAl ar simulated as a measure of the diffusion of sup 8 Li in the sample. As a possible time sequence for the measurement, a time cycle of 6s, i.e. the implantation of sup 8 Li for 1.5s and subsequent diffusion for 4.5s, is supposed. The sample is primarily set on a given temperature for the measurement. The time-dependent yields of alpha particles during the time cycle reveal the possibility to measure the diffusion coefficient with an accuracy of 10% if larger than 1 x 10 sup - sup 9 cm sup 2 /s, by the comparison with the experimental spectra measured at the temperature, i.e. at a certain diffusion coefficient. (author)

  3. Impact of short-lived non-CO2 mitigation on carbon budgets for stabilizing global warming

    International Nuclear Information System (INIS)

    Rogelj, Joeri; Riahi, Keywan; Meinshausen, Malte; Schaeffer, Michiel; Knutti, Reto

    2015-01-01

    Limiting global warming to any level requires limiting the total amount of CO 2 emissions, or staying within a CO 2 budget. Here we assess how emissions from short-lived non-CO 2 species like methane, hydrofluorocarbons (HFCs), black-carbon, and sulphates influence these CO 2 budgets. Our default case, which assumes mitigation in all sectors and of all gases, results in a CO 2 budget between 2011–2100 of 340 PgC for a >66% chance of staying below 2°C, consistent with the assessment of the Fifth Assessment Report of the Intergovernmental Panel on Climate Change. Extreme variations of air-pollutant emissions from black-carbon and sulphates influence this budget by about ±5%. In the hypothetical case of no methane or HFCs mitigation—which is unlikely when CO 2 is stringently reduced—the budgets would be much smaller (40% or up to 60%, respectively). However, assuming very stringent CH 4 mitigation as a sensitivity case, CO 2 budgets could be 25% higher. A limit on cumulative CO 2 emissions remains critical for temperature targets. Even a 25% higher CO 2 budget still means peaking global emissions in the next two decades, and achieving net zero CO 2 emissions during the third quarter of the 21st century. The leverage we have to affect the CO 2 budget by targeting non-CO 2 diminishes strongly along with CO 2 mitigation, because these are partly linked through economic and technological factors. (letter)

  4. Proceedings of the specialists' meeting on 'nuclear spectroscopy and condensed matter physics using short-lived nuclei'

    International Nuclear Information System (INIS)

    Kobayashi, Yoshio; Shibata, Michihiro; Ohkubo, Yoshitaka

    2016-02-01

    The research reactor at Research Reactor Institute, Kyoto University is a very useful neutron generator, providing us neutron-rich unstable nuclei by bombarding nuclei with those neutrons. The produced unstable nuclei exhibit aspects distinct from those of stable ones. Nuclear structure studies on a variety of excited states reflecting dynamic nuclear properties are one of fascinating research subjects of physics. On the other hand, some radioactive nuclei can be used as useful probes for understanding interesting properties of condensed matters through studies of hyperfine interactions of static nuclear electromagnetic moments with extranuclear fields. Concerning these two research fields and related areas, the 2nd symposium under the title of 'Nuclear Spectroscopy and Condensed Matter Physics Using Short-lived Nuclei' was held at the Institute for two days on November 4 and 5 in 2015. We are pleased that many hot discussions were made. The talks were given on the followings: 1) Nuclear spectroscopic experiments, 2) TDPAC (time-differential perturbed angular correlation), 3) β-NMR (nuclear magnetic resonance), 4) Moessbauer spectroscopy, 5) muon, etc. This issue is the collection of 17 papers presented at the entitled meeting. The 6 of the presented papers are indexed individually. (J.P.N.)

  5. Comparison of short-lived medical isotopes activation by laser thin target induced protons and conventional cyclotron proton beams

    Science.gov (United States)

    Murray, Joseph; Dudnikova, Galina; Liu, Tung-Chang; Papadopoulos, Dennis; Sagdeev, Roald; Su, J. J.; UMD MicroPET Team

    2014-10-01

    Production diagnostic or therapeutic nuclear medicines are either by nuclear reactors or by ion accelerators. In general, diagnostic nuclear radioisotopes have a very short half-life varying from tens of minutes for PET tracers and few hours for SPECT tracers. Thus supplies of PET and SPECT radiotracers are limited by regional production facilities. For example 18F-fluorodeoxyglucose (FDG) is the most desired tracer for positron emission tomography because its 110 minutes half-life is sufficient long for transport from production facilities to nearby users. From nuclear activation to completing image taking must be done within 4 hours. Decentralized production of diagnostic radioisotopes will be idea to make high specific activity radiotracers available to researches and clinicians. 11 C, 13 N, 15 O and 18 F can be produced in the energy range from 10-20 MeV by protons. Protons of energies up to tens of MeV generated by intense laser interacting with hydrogen containing targets have been demonstrated by many groups in the past decade. We use 2D PIC code for proton acceleration, Geant4 Monte Carlo code for nuclei activation to compare the yields and specific activities of short-lived isotopes produced by cyclotron proton beams and laser driven protons.

  6. Short-lived non-coding transcripts (SLiTs): Clues to regulatory long non-coding RNA.

    Science.gov (United States)

    Tani, Hidenori

    2017-03-22

    Whole transcriptome analyses have revealed a large number of novel long non-coding RNAs (lncRNAs). Although the importance of lncRNAs has been documented in previous reports, the biological and physiological functions of lncRNAs remain largely unknown. The role of lncRNAs seems an elusive problem. Here, I propose a clue to the identification of regulatory lncRNAs. The key point is RNA half-life. RNAs with a long half-life (t 1/2 > 4 h) contain a significant proportion of ncRNAs, as well as mRNAs involved in housekeeping functions, whereas RNAs with a short half-life (t 1/2 regulatory ncRNAs and regulatory mRNAs. This novel class of ncRNAs with a short half-life can be categorized as Short-Lived non-coding Transcripts (SLiTs). I consider that SLiTs are likely to be rich in functionally uncharacterized regulatory RNAs. This review describes recent progress in research into SLiTs.

  7. Investigation of short-lived neutron-rich palladium and silver isotopes after fast chemical separation from fission fragments

    International Nuclear Information System (INIS)

    Bruechle, W.

    1976-01-01

    In this paper, chemical separation processes are described permitting fast and neat isolation of short-lived palladium and silver nuclides from fusion product mixtures. The process for palladium is based on the stability of palladium diethyldithiophosphate. From fission products of the reactions 238 U(n,f) and 249 Cf(nth,f), the following palladium niclides could be studied for the first time by gamma spectroscopy: 1.66 min 113 Pd, 2.45 min 114 Pd, 29 sec sup(115a)Pd, 54 sec sup(115b)Pd, 12.5 sec 116 Pd. 113 Pd could also be indentified according to the reaction 116 Cd(n,α) 113 Pd. The separation of silver is based on the fast isotopic exchange on AgCl. With this process, the following nuclides have been separated from fission product mixtures and studied by gamma spectroscopy: 70 sec sup(113m)Ag, 5.0 sec 114 Ag, 19.2 sec sup(115m)Ag, 2.65 min sup(116g)Ag, 10.5 sec sup(116m)Ag, 1.3 min sup(117g)Ag, 6.0 sec sup(117m)Ag, 4.0 sec 118 Ag. (orig./WL) [de

  8. Plutonium, cesium and uranium series radionuclides in the Hudson River estuary and other environments. Annual technical progress report, 1 December 1980-30 November 1981

    International Nuclear Information System (INIS)

    Simpson, H.J.; Trier, R.M.

    1981-01-01

    Radionuclide activities were measured in sediment cores and suspended particle samples throughout the salinity range of the Hudson River estuary. Activities of 137 Cs, 134 Cs, 60 Co, 239 240 Pu, and 238 Pu indicate reasonably rapid accumulation rates in the sediments of marginal cove areas, and very rapid deposition in the harbor region adjacent to New York City, resulting in 239 240 Pu accumulations there more than an order of magnitude greater than the fallout delivery rate. Fallout 239 240 Pu reaching the Hudson is almost completely retained within the systems by particle deposition, while 80 to 90% of the 137 Cs derived from both reactor releases and fallout is exported to the coastal waters in solution. Depth profiles of radionuclides in Hudson sediments are not significantly altered by physical mixing processes in the sediments in areas accumulating particles at greater than 1 cm/yr. Measurements of fallout 239 2 xperimental quantities

  9. Estimate of whole body doses for Lynette Tew and Becky Farnsworth from Nevada Test Site local fallout

    International Nuclear Information System (INIS)

    Anspaugh, L.R.; Ng, Y.C.

    1985-01-01

    Lynette Tew and Becky Farnsworth are decendents whose relatives are litigants in Timothy vs US. The litigants allege that the decendents were harmed by radiation doses received as a result of local fallout from the testing of nuclear weapons at the Nevada Test Site. We have calculated a best estimate of the whole body dose received by each decendent from external exposure and the ingestion of radionuclides with food. In each case the dose via ingestion is trivial compared to the external dose. For Lynette Tew the dose estimate is 0.28 rads. For Becky Farnsworth it is 0.0035 rads. 23 references, 4 tables

  10. Radionuclides in the oceans inputs and inventories

    International Nuclear Information System (INIS)

    Guegueniat, P.; Germain, P.; Metivier, H.

    1996-01-01

    Ten years after Chernobyl, following the decision by France to end nuclear weapon testing in the Pacific ocean, after the end of the OECD-NEA Coordinated Research and Environmental Surveillance programme related to low-level waste dumping in the deep ocean, and one hundred years after the discovery of radioactivity, the IPSN wanted to compile and review the available information on artificial radioactivity levels in seas and oceans. International experts have been invited to present data on inputs and inventories of radionuclides in the marine environment, and to describe the evolution of radioactivity levels in water, sediments and living organisms. Different sources of radionuclides present in the aquatic environment are described: atmospheric fallout before and after Chernobyl, industrial wastes, dumped wastes and ships, nuclear ship accidents, river inputs, earth-sea atmospheric transfers and experimental sites for nuclear testing. Radioactivity levels due to these sources are dealt with at ocean (Atlantic, Pacific and Indian) and sea level (Channel, North Sea, Irish Sea, Mediterranean, Baltic, Black Sea and Arctic seas). These data collected in the present book give an up-to-date assessment of radionuclide distributions which will be very useful to address scientific and wider public concerns about radionuclides found in the aquatic environment. It gives many references useful to those who want to deepen their understanding of particular aspects of marine radioecology. (authors)

  11. Fallout radiation protection provided by transportation vehicles

    Energy Technology Data Exchange (ETDEWEB)

    Burson, Z.G.

    1972-10-20

    Fallout radiation protection factors (PF's) were estimated for a variety of civilian transportation vehicles using measurements of the natural terrain radiation as a source. The PF values are below 2 in light vehicles, truck beds, or trailers; from 2.5 to 3 in the cabs of heavy trucks and in a railway guard car; and from 3.0 to 3.5 in the engineer's seat of heavy locomotives. This information can be useful in planning the possible movement of personnel from or through areas contaminated either by a wartime incident or a peacetime accident. The information may also be useful for studying the reduction of exposure to the natural terrestrial radiation environment provided by vehicles.

  12. 111Ag in the Chernobyl fallout

    International Nuclear Information System (INIS)

    Winkler, R.; Rosner, G.; Hoetzl, H.

    1989-01-01

    In the course of a re-evalution of the gamma-ray spectra of air filter samples collected immediately after Chernobyl accident at Munich-Neuherberg 111 Ag has been found to contribute significantly to the total activity within the first days of the Chernobyl fallout. The maximum air concentration was measured on 1 May 1986 to be 5.4 Bq/m 3 compared with 9.7 Bq 137 Cs per m 3 . Referred to this date the total activity deposition to ground was 12±3 kBq 111 Ag per m 2 . Referred to 26 April 1986 the 111 Ag to 110m Ag ratio was found to be 53±3 and the 111 Ag to 137 Cs ratio was 1.0±0.1. It is estimated that the cesium isotopes were depleted during release and atmospheric transport by a factor of about 2 compared with the silver isotopes. (orig.)

  13. Methodology for determination of activity of radionuclides by gamma spectrometry

    International Nuclear Information System (INIS)

    Fragoso, Maria da Conceicao de Farias; Oliveira, Victor Rogerio S. de; Oliveira, Mercia L.; Lima, Fernando Roberto de Andrade

    2014-01-01

    Due to the growth in the number of procedures that make use of the positron emission tomography (PET), there is a need for standard solutions for the calibration of the systems used for the measurement of the PET radiopharmaceutical (activimeter) in radiopharmacies and in nuclear medicine services. Among the existing alternatives for the standardization of radioactive sources, the method known as gamma spectrometry is widely used for short-lived radionuclides. The purpose of this study was to implement the methodology for standardization of the 18 F solutions by gamma spectrometry at the Regional Center for Nuclear Sciences of the Northeast (CRCN-NE/CNEN-NE), Brazil. (author)

  14. Cyclotron production of molecules labelled with short-lived radioisotopes β+ emitters (15O, 13N, 11C) and their clinical uses

    International Nuclear Information System (INIS)

    Bougharouat, B.

    1981-01-01

    Clinical use of three short-lived radioisotopes: 15 O, 13 N and 11 C is studied on two complementary aspects. A production and purification system is realized; detection instruments in medical use are studied. The production of labelled molecules with the three radiotracers 15 O, 13 N, 11 C from the target bombardment with charged and accelerated particles was studied [fr

  15. A crossed-beam experiment on intramultiplet mixing collisions with short-lived Ne** {(2p)5(3p)} atoms

    NARCIS (Netherlands)

    Manders, M.P.I.; Ruyten, W.M.J.; van de Beucken, F..J.H.M.; Driessen, J.P.J.; Veugelers, W.J.T.; Kramer, P.H.; Vredenbregt, E.J.D.; van Hoek, W.B.M.; Sandker, G.J.; Beijerinck, H.C.W.; Verhaar, B.J.

    1988-01-01

    We describe the design, operation, and calibration of a crossed-beam experiment for the study of intramultiplet mixing collisions of short-lived electronically excited Ne{(2p)5(3p)}≡{α} atoms with ground-state atoms/molecules. The excellent performance of almost 1 kHz/Å2 (number of counts per unit

  16. Transport and deposition of nano-particles. Application to the free action of short-lived radon daughters; Transport et depot des aerosols nanometriques. Application a la fraction libre des descendants a vie courte du radon

    Energy Technology Data Exchange (ETDEWEB)

    Malet, J

    1997-10-10

    Short-lived radon daughters ({sup 218}Po, {sup 214}Pb, {sup 214}Bi, and {sup 214}Po) are important contributors to the natural average annual individual dose. The models describing the evolution of these aerosol in a house depend critically on a parameter, the {sup 218}Po deposition velocity, which, although aerosol deposition has been extensively studied, is poorly known. A numerical and experimental study is thus carried out for a simple case: deposition in a cylindrical tube under laminar flow condition. The numerical results help understanding the difference between the transport and deposition of these radionuclides and those of non radioactive aerosols. Comparison of these well environment does not give satisfactory correlation, requiring the study of phenomena that may affect deposition. The first of these is the possible variation in the e {sup 218}Po diffusion coefficient. Furthermore, experiments coupled with numerical calculations show that this variation could be due to {sup 218}Po neutralization. The second phenomenon concerns the effect of the surface type, which is also shown experimentally. By modelling the neutralization and using results with a piratically smooth surface, good numerical/experimental correlations are obtained. Understanding this simple case than makes possible studying a more complex case: deposition in controlled turbulent flow. Two theories are thus experimentally validated. In addition, a {sup 218}Po deposition velocity representative of our experimental conditions is determined. Finally, we report a feasibility study of radon daughters transport and deposition in a ventilated chamber taking into account all the involved phenomena. (author)

  17. Radionuclide sources in the Barents and Kara Seas

    International Nuclear Information System (INIS)

    Smith, J.N.; Ellis, K.M.; Forman, S.; Polyak, L.; Ivanov, G.; Matishov, D.; Kilius, L.

    1995-01-01

    A study of radionuclide distributions in the Barents Sea sediments was carried out in 1992. The conclusions of the study are as follows: 1) Elevated levels of artificial radionuclides as great as 15,000 Bq/kg for 239,240 Pu, 250 Bq/kg for 137 Cs and 100 Bq/kg for 60 Co were measured in sediments in Chermaya Bay which have been contaminated by several nuclear tests conducted in the 1950s. 2) Sediment-depth distributions of 239,240 Pu and other artificial radionuclides are consistent with results from biodiffusion models that are constrained by 210 Pb sediment-depth distributions. These results indicate that sedimentation rates in Chernaya Bay are low ( 249 Pu/ 239 Pu and 241 Pu/ 239 Pu atom ratios of 0.030 and 0.0012, respectively and a 241 Am/ 239,240 Pu activity ratio of 0.05 (compared to 0.3 in fallout) which provides a method for tracking its dispersion over distances of 100 km into the Barents Sea. 4) Artificial radionuclide levels in sediments and seawater near a sunken barge loaded with radioactive wastes in the Novaya Zemlya trough are similar to background fallout levels in the Kara Sea and provide little evidence for the release of radioactive contaminants from the dumpsite. 7 refs., 4 figs

  18. Ecological processes in the cycling of radionuclides within arctic ecosystems

    International Nuclear Information System (INIS)

    Hanson, W.C.

    1986-01-01

    Worldwide fallout radionuclides in arctic ecosystems was investigated ecologically by circumpolar nations during 1959-80. Several of the radionuclides are isotopes of elements which currently contribute to arctic haze; they thus serve as effective tracers of biogeochemical processes. Investigations demonstrated the effective concentration of several radionuclides, particularly strontium-90 (an alkaline earth metal) and cesium-137 (a light alkali metal) which are chemical analogs of calcium and potassium, two very important stable elements in biotic systems. Transfer of 137 Cs through the lichen-cariboureindeer-man food chain characteristic of circumpolar nations, resulted in body burdens in Inuit that were 20 to 200 times greater than those in human populations of temperature latitudes. Radiation exposures from 90 Sr, 137 Cs and other natural and worldwide fallout radionuclides, were two to three times greater than for most other world populations. These results demonstrate the concentration capabilities of arctic ecosystems for several groups of chemical elements that have counterparts in arctic haze. These elements, therefore, provide the basis for considering the ecological implications of current situations

  19. Radioactive fallout in air and rain: results to the end of 1990

    International Nuclear Information System (INIS)

    Playford, K.; Lewis, G.N.J.; Carpenter, R.C.

    1992-01-01

    Samples of atmospheric particulate and rainwater have been collected from the United Kingdom and elsewhere. Results are presented of analyses of these samples for various fission products and certain other radionuclides. Average concentrations of Cs-137 in air in the United Kingdom in 1990 were 1% of those in 1986. They were attributable mainly to the resuspension of deposited activity resulting from the Chernobyl accident of April 1986. Plutonium concentrations in air and rainwater were a very small fraction of the National Radiological Protection Board's Generalised Derived Limit for members of the public. Estimates are given of the worldwide deposit of Cs-137 and Sr-90 to the end of 1990. The gamma and beta-ray dose rates from fallout at Chilton are estimated from the observed deposition. (author)

  20. Chernobyl fallout in Greece and its effects on the dating of archaeological materials

    Energy Technology Data Exchange (ETDEWEB)

    Liritzis, Y

    1987-10-15

    The effects of the fallout from the nuclear reactor accident at Chernobyl have been monitored at various sites in Greece. Here we present the first estimates of gamma dose rates, an essential parameter in the dating of archaeological materials by thermoluminescence (TL) and ESR methods. The dose rates are derived from the long-lived radionuclides of /sup 137/Cs, /sup 134/Cs, /sup 106/Ru and /sup 144/Ce (with t/sub 1/2/ greater than or equal to 1 yr). The present dose rates vary between 30 and 60 mrad/yr, but maximum values of around 811 mrad/yr have also been recorded, for ground-surface exposures. These dose rate values must be regarded as very significant to TL and ESR dating of samples from now on and a correction factor should be applied.

  1. Evaluation of food contamination and health risks due to the radioactive fallout 90Sr before 2010

    International Nuclear Information System (INIS)

    Shimada, Yoko; Morisawa, Shinsuke

    2013-01-01

    Before the Fukushima Daiichi nuclear power plant accident, radionuclides like 90 Sr released by atmospheric nuclear detonation tests and the Chernobyl accident have been transported worldwide in the environment and finally taken up by humans through various pathways. In this research, the health risks caused by the prolonged exposure to fallout 90 Sr through food ingestion pathways were evaluated age-dependently for the reference Japanese since 1945 until 2010, using the mathematical model for evaluating global distribution of 90 Sr with food ingestion considering the domestic and international food supply in Japan. The model estimates were compared with the monitoring data of 90 Sr in Japanese total diet and 90 Sr concentration in food to examine the model validity. The results of this evaluation would be useful for understanding the background situations without the Fukushima accident and give important knowledge for the radiological health risk assessment of this accident. (author)

  2. The Chernobyl fallout in Greece and its effects on the dating of archaeological materials

    International Nuclear Information System (INIS)

    Liritzis, Y.

    1987-01-01

    The effects of the fallout from the nuclear reactor accident at Chernobyl have been monitored at various sites in Greece. Here we present the first estimates of gamma dose rates, an essential parameter in the dating of archaeological materials by thermoluminescence (TL) and ESR methods. The dose rates are derived from the long-lived radionuclides of 137 Cs, 134 Cs, 106 Ru and 144 Ce (with t 1/2 ≥ 1 yr). The present dose rates vary between 30 and 60 mrad/yr, but maximum values of around 811 mrad/yr have also been recorded, for ground-surface exposures. These dose rate values must be regarded as very significant to TL and ESR dating of samples from now on and a correction factor should be applied. (orig.)

  3. Inactivation of Candida glabrata by a humid DC argon discharge afterglow: dominant contributions of short-lived aqueous active species

    International Nuclear Information System (INIS)

    Xiong, Qing; Liu, Hongbin; Xu, Le; Wang, Xia; Zhu, Qunlin; Lu, Weiping; Chen, Qiang; Zeng, Xue; Yi, Ping

    2017-01-01

    Plasma medicine applications are currently attracting significant interest all over the world. Bactericidal treatments of Candida glabrata cultured in saline suspension are performed in this study by a room-temperature reactive afterglow of a DC-driven argon discharge. Water vapor was added to the discharge to study the inactivation contributions of reactive hydrolytic species including OH and H 2 O 2 transporting along the gas flow to the treated solutions. The inactivation results indicate that the dominant roles in the bactericidal treatments are played by the short-lived aqueous active species, but not the stable species like H 2 O 2aq (aq indicates an aqueous species). Further analysis shows that the ·OH aq radicals play an important role in the inactivation process. The ·OH aq radicals in the suspension are mostly produced from the direct dissolution of the OH species in the reactive afterglow. With the increase of added water vapor content, the ·OH aq production increases and enhances the inactivation efficiency of C. glabrata . Furthermore, it is found that the ambient air diffusion shows essential effects on the bactericidal activity of the remote humid argon discharge. Higher bactericidal effects can be obtained in open-space treatments compared to in a controlled Ar + H 2 O gas atmosphere. Key active air-byproduct species are believed to be generated in the suspension during the treatments and contributing to the inactivation process. Based on chemical analysis, the peroxynitrous acid ONOOH aq is considered as the key antimicrobial air-byproduct species. These results indicate the important dependence of plasma biomedical effects on the processing environment, which finally relates to the critical contributions of the key reactive species formed therein. (paper)

  4. Study on the risk of late damage in humans after incorporation of the short-lived alpha emitter Ra-224

    International Nuclear Information System (INIS)

    Wick, R.R.; Nekolla, E.A.; Kellerer, A.M.; Goessner, W.

    2003-01-01

    An epidemiological study has been carried out at the GSF - National Research Center for Environment and Health - between 1948 and 1975, on 1460 ankylosing spondylitis (AS) patients. The aim of the study was to ascertain the late health effects suffered by these patients who had received repeated intravenous injections of the short lived α-emitter 224 Ra. These patients have been followed together with a control group of 1323 ankylosing spondylitis patients not treated with radioactive drugs and/or X-rays. Causes of death have been ascertained for 842 exposed patients and 861 controls by the end of 2002. In the exposed group there has been a total of 219 malignant diseases and 206 cases among the controls. In particular, we observed 15 cases of leukaemia in the exposure group and 8 cases of leukaemia in the control group. Further subclassification of the leukaemias demonstrated a high increase of myeloid leukaemia in the exposure group (9 cases obs. vs. 2.5 cases exp.), and out of these especially the acute myeloid leukaemias (6 cases observed vs. 1.6 expected), whereas in the control group the observed cases are within the expected range (3 myeloid leukaemias vs. 2.6 cases). Out of these 6 cases of myeloid leukaemia, 3 cases have been observed at doses comparable to those of the currently applied 224 Ra treatment with the preparation SpondylAT registered , in one case the 224 Ra-dose was the 0.6fold, in another case 1.6fold, whereas in one case the total dose could not be verified exactly. The enhanced leukaemia incidence in our exposed group is in line with results from animal experiments in mice having been injected with bone seeking α-emitters given at low dose rates. (orig.) [de

  5. Inactivation of Candida glabrata by a humid DC argon discharge afterglow: dominant contributions of short-lived aqueous active species

    Science.gov (United States)

    Xiong, Qing; Liu, Hongbin; Lu, Weiping; Chen, Qiang; Xu, Le; Wang, Xia; Zhu, Qunlin; Zeng, Xue; Yi, Ping

    2017-05-01

    Plasma medicine applications are currently attracting significant interest all over the world. Bactericidal treatments of Candida glabrata cultured in saline suspension are performed in this study by a room-temperature reactive afterglow of a DC-driven argon discharge. Water vapor was added to the discharge to study the inactivation contributions of reactive hydrolytic species including OH and H2O2 transporting along the gas flow to the treated solutions. The inactivation results indicate that the dominant roles in the bactericidal treatments are played by the short-lived aqueous active species, but not the stable species like H2O2aq (aq indicates an aqueous species). Further analysis shows that the ·OHaq radicals play an important role in the inactivation process. The ·OHaq radicals in the suspension are mostly produced from the direct dissolution of the OH species in the reactive afterglow. With the increase of added water vapor content, the ·OHaq production increases and enhances the inactivation efficiency of C. glabrata. Furthermore, it is found that the ambient air diffusion shows essential effects on the bactericidal activity of the remote humid argon discharge. Higher bactericidal effects can be obtained in open-space treatments compared to in a controlled Ar + H2O gas atmosphere. Key active air-byproduct species are believed to be generated in the suspension during the treatments and contributing to the inactivation process. Based on chemical analysis, the peroxynitrous acid ONOOHaq is considered as the key antimicrobial air-byproduct species. These results indicate the important dependence of plasma biomedical effects on the processing environment, which finally relates to the critical contributions of the key reactive species formed therein.

  6. Biological accessibility of Chernobyl radionuclides and aspects of environmental rehabilitation

    International Nuclear Information System (INIS)

    Sokolik, G.A.; Leinova, S.L.; Ivanova, T.G.; Duksina, V.V.; Rubinchik, S.Ya.; Zaharenkov, V.V.

    1998-01-01

    The redistribution of 137 Cs, 90 Sr, 239,240 Pu and 241 Am within natural ecosystems and the determination of natural and artificial factors influencing on processes of radionuclide migration on biogeochemical chains were investigated. There are three main directions of investigation. The first of them is to estimate the intensity of self-purification of damaged region soil cover, taking into account landscape, soil, land-use differentiation and also peculiarities of physico-chemical occurrence forms of the radioactive fallout. In particular, the change dynamics of radionuclide physico-chemical state and vertical migration in soil of different genesis were estimated, the soil varieties with high and low rate of radionuclide migration were discovered, the peculiarities of 'hot' particles destruction, the change of their dispersity and structure composition under the influence of natural reagents were studied, the radionuclide bond strength with some components of different soil types was determined. The second problem is to estimate the biological accessibility of radionuclides. In particular, the radionuclide contamination of different components of forest and meadow phytocenoses was investigated, the change of radionuclide accumulation coefficients in system 'soil-plant' was estimated. The third problem is ecological and practice measures for environmental rehabilitation. In particular, the soil self-purification hypothesis in different natural conditions were created and the permissible criterion's of interference in natural processes were developed

  7. Radionuclide accumulation in fruit bodies of macromycetes

    International Nuclear Information System (INIS)

    Fedorov, V.N.; Eliashevich, N.V.

    2000-01-01

    By materials of the observation net within the limits of the Byelorussian sector of the ChNPP 30-rm zone (contamination up to 16.65 MBq/m 2 ) the radioactivity was considered at the territories with the background contamination (up to 37 kBq/m 2 ), at the South-Bobrujsk (up to 185 kBq/m 2 ) and Volozhinsk (up to 555 kBq/m 2 ) fallout spots. The accumulation and proportionality coefficients of 137 Cs in 36 species and 90 Sr in 19 species of macromycetes of various tropic groups under the drought y year conditions, their changeability by forest formations and in the time within the range of 1992-1998 are determined. The average two-fold increase in the species contamination a year with increased atmospheric humidity (1998) is indicated. The closer contamination correlation of the Boletus edulis with photosynthetically active part of the Betula pendula and Pinus sylvestris, as compared to the soil pollution, shows the possibility of indicating the pollution of short-living fruit bodies of fungi by the pollution of the plants-symbiotrophs [ru

  8. Evaluation of the uncertainty around the mean level of 137Cs fallout at undisturbed reference site: A simple statistical approach

    International Nuclear Information System (INIS)

    Mabit, L.; Gonsalves, B.C.; Chen, X.; Toloza, A.; Weltin, G.; Darby, I.G.; Padilla-Alvarez, R.

    2015-01-01

    One of the major issues related to the use of 137 Cs as a soil erosion/sedimentation tracer is the selection of the reference site which is used to estimate the initial 137 Cs fallout input (also termed reference inventory). The initial 137 Cs fallout input is a key component of the conversion models used to estimate erosion and sedimentation rates from the 137 Cs data set. The selection and evaluation of the validity of reference sites have been explained in detail in the recent IAEA TECDOC 1741 ‘‘Guidelines for using Fallout radionuclides to assess erosion and effectiveness of soil conservation strategies’’. An investigation was carried out at the experimental research station of the Austrian Agency for Health and Food Safety (AGES), in Austria, Grabenegg (48°07'40 N , 15°13'16 E ). Located at an altitude of 260 m a.s.l, with an annual average temperature of 8.4 °C and annual precipitation of 686 mm, the soil of this area has been classified as Gleyic Cambisol with a silt-loamy texture

  9. A multi-radionuclide approach to evaluate the suitability of 239+240Pu as soil erosion tracer

    International Nuclear Information System (INIS)

    Meusburger, Katrin; Mabit, Lionel; Ketterer, Michael; Park, Ji-Hyung; Sandor, Tarjan; Porto, Paolo; Alewell, Christine

    2016-01-01

    Fallout radionuclides have been used successfully worldwide as tracers for soil erosion, but relatively few studies exploit the full potential of plutonium (Pu) isotopes. Hence, this study aims to explore the suitability of the plutonium isotopes 239 Pu and 240 Pu as a method to assess soil erosion magnitude by comparison to more established fallout radionuclides such as 137 Cs and 210 Pb ex . As test area an erosion affected headwater catchment of the Lake Soyang (South Korea) was selected. All three fallout radionuclides confirmed high erosion rates for agricultural sites (> 25 t ha −1 yr −1 ). Pu isotopes further allowed determining the origin of the fallout. Both 240 Pu/ 239 Pu atomic ratios and 239+240 Pu/ 137 Cs activity ratios were close to the global fallout ratio. However, the depth profile of the 239+240 Pu/ 137 Cs activity ratios in undisturbed sites showed lower ratios in the top soil increments, which might be due to higher migration rates of 239+240 Pu. The activity ratios further indicated preferential transport of 137 Cs from eroded sites (higher ratio compared to the global fallout) to the depositional sites (smaller ratio). As such the 239+240 Pu/ 137 Cs activity ratio offered a new approach to parameterize a particle size correction factor that can be applied when both 137 Cs and 239+240 Pu have the same fallout source. Implementing this particle size correction factor in the conversion of 137 Cs inventories resulted in comparable estimates of soil loss for 137 Cs and 239+240 Pu. The comparison among the different fallout radionuclides highlights the suitability of 239+240 Pu through less preferential transport compared to 137 Cs and the possibility to gain information regarding the origin of the fallout. In conclusion, 239+240 Pu is a promising soil erosion tracer, however, since the behaviour i.e. vertical migration in the soil and lateral transport during water erosion was shown to differ from that of 137 Cs, there is a clear need for a

  10. Baltic Sea: Radionuclides

    DEFF Research Database (Denmark)

    Nielsen, Sven Poul; Lüning, Maria; Ilus, Erkki

    2011-01-01

    The most significant source of anthropogenic radioactivity in the Baltic Sea is fallout from the accident at the Chernobyl nuclear power plant in 1986. The second most important source is global fallout from atmospheric nuclear weapons tests carried out during the late 1950s and early 1960s...... about 14%. For 90Sr in the Baltic Sea, input from atmospheric fallout from nuclear weapons tests has contributed about 81%, while the contribution from Chernobyl fallout was about 13%. Cesium-137 is the main indicator of Baltic seawater with respect to anthropogenic radioactivity. The highest...... concentrations in seawater during 1999–2006 were found in the Baltic Proper and the Bothnian Sea. The general trend is steadily decreasing. Concentrations of anthropogenic radioactivity in fish generally show decreasing trends in agreement with concentrations in seawater. Among freshwater fish, pike showed large...

  11. Baltic Sea: Radionuclides

    DEFF Research Database (Denmark)

    Nielsen, Sven Poul; Lüning, Maria; Ilus, Erkki

    2010-01-01

    The most significant source of anthropogenic radioactivity in the Baltic Sea is fallout from the accident at the Chernobyl nuclear power plant in 1986. The second most important source is global fallout from atmospheric nuclear weapons tests carried out during the late 1950s and early 1960s...... about 14%. For 90Sr in the Baltic Sea, input from atmospheric fallout from nuclear weapons tests has contributed about 81%, while the contribution from Chernobyl fallout was about 13%. Cesium-137 is the main indicator of Baltic seawater with respect to anthropogenic radioactivity. The highest...... concentrations in seawater during 1999–2006 were found in the Baltic Proper and the Bothnian Sea. The general trend is steadily decreasing. Concentrations of anthropogenic radioactivity in fish generally show decreasing trends in agreement with concentrations in seawater. Among freshwater fish, pike showed large...

  12. Biomedical research and application utilizing cyclotron produced radionuclides. Progress report, January 1 1977--December 31, 1977

    International Nuclear Information System (INIS)

    Laughlin, J.S.; Benua, R.S.; Tilbury, R.S.

    1977-01-01

    Progress is reported on cyclotron production of short-lived positron-emitting radionuclides ( 18 F, 15 O, 11 C, 13 N, 52 Fe, 38 K, 206 Bi, 73 Se, and 48 Cr) for use in the preparation labelled compounds for metabolic research in patients and animals. The chemical preparation of radiopharmaceuticals labelled with cyclotron-produced radionuclides for pancreas and tumor scanning is discussed. The imaging capabilities of a total organ kinetic imaging monitor (TOKIM) gamma camera system operated in the positron coincidence mode were improved with the addition of computerized iterative correction procedures

  13. Implementation of sum-peak method for standardization of positron emission radionuclides

    International Nuclear Information System (INIS)

    Fragoso, Maria da Conceicao de Farias; Oliveira, Mercia Liane de; Lima, Fernando Roberto de Andrade

    2015-01-01

    Positron Emission Tomography (PET) is being increasingly recognized as an important quantitative imaging tool for diagnosis and assessing response to therapy. As correct dose administration plays a crucial part in nuclear medicine, it is important that the instruments used to assay the activity of the short-lived radionuclides are calibrated accurately, with traceability to the national or international standards. The sum-peak method has been widely used for radionuclide standardization. The purpose of this study was to implement the methodology for standardization of PET radiopharmaceuticals at the Regional Center for Nuclear Sciences of the Northeast (CRCN-NE). (author)

  14. Radionuclides in animal tissue samples from various regions of Austria

    International Nuclear Information System (INIS)

    Tatzber, F.

    1981-06-01

    An investigation of the concentration of radioactive substances in animal species from various regions of Austria has been carried out. For bone and liver of deer, radionuclide concentrations typical for central Europe were found. The content of 90 Sr were higher in gasteropod shells than in deer bone. Similar concentrations of 90 Sr were found in isopods as in snail shells related to fresh weight, but related to Ca content the values in isopods were higher than in all other animals. Based on these results, a study of snail shells and of isopods as bioindicators for 90 Sr content in environmental control is indicated. In tissue samples of the same species, but from different regions of Austria, the fallout radionuclide concentrations were found to be related to altitude ( 90 Sr) and to the amount of precipitation ( 137 Cs). These correlation differences could point to a different deposition behaviours of 90 Sr and 137 Cs, the former being deposited mainly with solid precipitation. This seems plausible since aerosols carried over continental distances show a high sulfate content and alkaline earth metal sulfates are less soluble than alkali sulfates. Examination of absolute concentration values related to fresh tissue weight show high fallout radionuclide concentrations, as compared to natural radionuclide concentration, especially in hard tissues. These fallout levels constitute a significant radioactive load on the biosphere. Due to the long physical half-life of 90 Sr and 137 Cs, this situation will remain virtually unchanged during the next decades, even if no further nuclear weapons tests are carried out. (G.G.)

  15. The effects of the marine biosphere and hydrosphere upon the specific activity of contaminant radionuclides

    International Nuclear Information System (INIS)

    Lowman, F.G.

    1969-01-01

    Fusion and fission products as well as neutron induced radionuclides will be produced by the use of nuclear explosives for excavation. Stable elements from the geological matrix which are vaporized at the time of detonation will be vented in the same form as the radionuclides and will dilute the radionuclides to different specific activities depending upon the yield and design of the explosive, the neutron flux, neutron cross-sections for the stable elements and the homogeneity of the rock. Radionuclides in the cloud and fallout may be further diluted by pulverized rock on which they plate although the chemical forms may or may not be the same. This fallout material may be deposited into the sea and will react with sea water and its contained salts to precipitate or co-precipitate some radionuclides and release others as colloids or solutes where they will be subject to further dilution by the stable elements in sea water. The radionuclides will be subjected to varying amounts of physical and chemical dilution according to the physical environmental parameters. In some estuarine and upwelling areas of high biological productivity, the radionuclides and corresponding stable elements may become incorporated into cycles involving the biosphere, hydrosphere and bottom sediments in which the added material will remain in the area for longer periods of time than that expected from physical mixing and dilution. (author)

  16. The effects of the marine biosphere and hydrosphere upon the specific activity of contaminant radionuclides

    Energy Technology Data Exchange (ETDEWEB)

    Lowman, F G [Puerto Rico Nuclear Center, Mayaguez (Puerto Rico)

    1969-07-01

    Fusion and fission products as well as neutron induced radionuclides will be produced by the use of nuclear explosives for excavation. Stable elements from the geological matrix which are vaporized at the time of detonation will be vented in the same form as the radionuclides and will dilute the radionuclides to different specific activities depending upon the yield and design of the explosive, the neutron flux, neutron cross-sections for the stable elements and the homogeneity of the rock. Radionuclides in the cloud and fallout may be further diluted by pulverized rock on which they plate although the chemical forms may or may not be the same. This fallout material may be deposited into the sea and will react with sea water and its contained salts to precipitate or co-precipitate some radionuclides and release others as colloids or solutes where they will be subject to further dilution by the stable elements in sea water. The radionuclides will be subjected to varying amounts of physical and chemical dilution according to the physical environmental parameters. In some estuarine and upwelling areas of high biological productivity, the radionuclides and corresponding stable elements may become incorporated into cycles involving the biosphere, hydrosphere and bottom sediments in which the added material will remain in the area for longer periods of time than that expected from physical mixing and dilution. (author)

  17. Nevada Test Site fallout in the area of Enterprise, Utah

    International Nuclear Information System (INIS)

    Krey, P.W.; Hardy, E.P.; Heit, M.

    1980-04-01

    The analysis of a sediment core from the Enterprise reservoir in southwestern Utah has provided a record of fallout in the area dating to 1945. Assming that all the 137 Cs fallout that occurred at Enterprise reservoir between 1951 and 1957 came exclusively from the Nevada tests, an upper limit of the integrated deposit from this source is 18 mCi/km 2 of 137 Cs decay corrected to 1979 out of a total of 101 measured in 1979. The maximum infinity dose from the external radiation caused by this Nevada Test Site fallout is estimated to be 1700 mrad. This maximum dose is only a factor of two higher than the cumulative estimated dose in Enterprise derived from the radiological surveys conducted after each test. This indicates that the region around Enterprise reservoir did not experience an intrusion of fallout from NTS greatly in excess of what had been deduced from the post-shot external radiation surveys

  18. The biological transport of radionuclides in grassland and freshwater ecosystems

    International Nuclear Information System (INIS)

    Rudge, S.A.

    1989-12-01

    This thesis examines the biological transport of radionuclides through terrestrial and aquatic ecosystems, with particular reference to radiocaesium. The semi-natural grassland habitat was located at Drigg, W. Cumbria, contaminated primarily by radioactive fallout, from several sources over the past decade. Advantage was made of the deposition of radionuclides from the Chernobyl reactor incident, which occurred during the early stages of the investigation. The study examined the distribution of radiocaesium for the major components of the grassland ecosystem, within the soil-plant-invertebrate-small mammal food chain. Data concerning temporal fluctuation of radionuclide transfer factors between food chain components are presented. The final section examines the spatial distribution of radiocaesium in sediment and the freshwater eel (Anguilla anguilla) in a small stream contaminated by radioactive effluent. The relationship between activity levels in eels and the sediments in which they rest and forage was investigated. Factors influencing uptake of radiocaesium in freshwater fish were also examined. (author)

  19. Local fall-out and the animal food chain; Retombees locales et chaine alimentaire animale

    Energy Technology Data Exchange (ETDEWEB)

    Prat, G.; Mercier, F.J. [Commissariat a l' Energie Atomique, Fontenay-aux-Roses (France). Centre d' Etudes Nucleaires

    1967-07-01

    The local consequences of fresh fall-out, especially in the case of atmospheric nuclear explosions, are reviewed from the point of view of the internal contamination of the consumer of foodstuffs of animal origin. The edibility of foodstuffs derived from animals having grazed in the presence of fall-out is evaluated both from the wholesome and radio-toxicological points of view. The contamination level of these foodstuffs is calculated as a function of the ground fall-out, and of agronomical and ecological parameters for each radio-nuclide of the animal food chain. The internal exposure of the human consumer is calculated from this level as a function of the diet and of various parameters especially temporal. The equivalent dose to each critical organ, including the digestive tract is deduced from the burdens of each organ. From this a nutritional hygiene in the areas affected by fall-out is obtained, in relationship to the action levels fixed by the responsible authorities in exceptional circumstances. Criteria for these action levels are given as function of the food rations. (authors) [French] Les consequences locales des retombees fraiches, notamment dans le cas d'explosions nucleaires atmospheriques, sont passees en revue en ce qui concerne les problemes de contamination interne du consommateur de denrees d'origine animale. La comestibilite des aliments provenant de betes de boucherie ayant pature sous les retombees est evaluee au double point de vue de la salubrite et de la radiotoxicologie. Le niveau de contamination de ces denrees est calcule en fonction de la retombee au sol, des parametres agronomiques et ecologiques pour chaque radioelement de la chaine alimentaire animale. La contamination interne du consommateur humain est calculee a partir de ce niveau en fonction des modalites d'ingestion et de divers parametres, notamment temporels. L'equivalent de dose au niveau de chaque organe critique, y compris le tube digestif, est deduit

  20. Local fall-out and the animal food chain; Retombees locales et chaine alimentaire animale

    Energy Technology Data Exchange (ETDEWEB)

    Prat, G; Mercier, F J [Commissariat a l' Energie Atomique, Fontenay-aux-Roses (France). Centre d' Etudes Nucleaires

    1967-07-01

    The local consequences of fresh fall-out, especially in the case of atmospheric nuclear explosions, are reviewed from the point of view of the internal contamination of the consumer of foodstuffs of animal origin. The edibility of foodstuffs derived from animals having grazed in the presence of fall-out is evaluated both from the wholesome and radio-toxicological points of view. The contamination level of these foodstuffs is calculated as a function of the ground fall-out, and of agronomical and ecological parameters for each radio-nuclide of the animal food chain. The internal exposure of the human consumer is calculated from this level as a function of the diet and of various parameters especially temporal. The equivalent dose to each critical organ, including the digestive tract is deduced from the burdens of each organ. From this a nutritional hygiene in the areas affected by fall-out is obtained, in relationship to the action levels fixed by the responsible authorities in exceptional circumstances. Criteria for these action levels are given as function of the food rations. (authors) [French] Les consequences locales des retombees fraiches, notamment dans le cas d'explosions nucleaires atmospheriques, sont passees en revue en ce qui concerne les problemes de contamination interne du consommateur de denrees d'origine animale. La comestibilite des aliments provenant de betes de boucherie ayant pature sous les retombees est evaluee au double point de vue de la salubrite et de la radiotoxicologie. Le niveau de contamination de ces denrees est calcule en fonction de la retombee au sol, des parametres agronomiques et ecologiques pour chaque radioelement de la chaine alimentaire animale. La contamination interne du consommateur humain est calculee a partir de ce niveau en fonction des modalites d'ingestion et de divers parametres, notamment temporels. L'equivalent de dose au niveau de chaque organe critique, y compris le tube digestif, est deduit des charges de ces

  1. Excitation functions for the formation of some short-lived products in proton-induced reactions on silver

    OpenAIRE

    Uddin, M. S.; Baba, M.; Hagiwara, M.; Latif, S. K. A.; Qaim, S. M.

    2008-01-01

    Excitation functions of the Ag-nat(p, xn)Cd-104,Cd-105 and Ag-nat(p, pxn) Ag-103,Ag-104m.g,Ag- 1049 reactions were measured for the first time over the proton energy range of 32 to about 60 MeV. The data were compared with the results of precompound-hybrid model calculations, whereby only partial agreement was obtained. The contribution of the Ag-103 precursor decay to the total formation of the therapeutic radionuclide Pd-103 in proton activation of silver was estimated: it amounted to about...

  2. gamma. -spectra of radioactive fallout from the atmosphere. [In German

    Energy Technology Data Exchange (ETDEWEB)

    Herbst, W; Sommermeyer, K

    1957-01-01

    Foils used for collecting dust which were exposed to radioactive fallout for 8 days, and grass ashes exhibit the same ..gamma..-spectra. The peaks were characteristic of the following isotopes, half-lives in brackets: /sup 140/Ba (13 days) + /sup 140/La; /sup 95/Zr (65 days) + /sup 95/Nb; and /sup 103/Ru (40 days). Relative peak heights indicated age of fallout.

  3. Impact of fallout from Chernobyl on Saclay site

    International Nuclear Information System (INIS)

    1986-07-01

    The fallout from Chernobyl accident have been monitored at Saclay Nuclear Research Center. The initial results from external irradiation measurement and analysis of environmental samples: air, fallout deposits, surface water, drinking water, underground water, food chain, are presented. The population radiation doses from external exposure to the plume, inhaled radioactivity and consumption of meat, milk and vegetables have been estimated. Special monitoring of internal contamination by iodine 131, cesium 134 and cesium 137 has been carried out using whole body counting [fr

  4. Childhood leukemias associated with fallout from nuclear testing

    International Nuclear Information System (INIS)

    Lyon, J.L.; Klauber, M.R.; Gardner, J.W.; Udall, K.S.

    1979-01-01

    Continuing concern over the possible carcinogenic effects of low-level radiation prompted us to study the population of Utah because of its exposure to fallout from 26 nuclear tests between 1951 and 1958. Certain rural counties (high-level counties) received most of the fallout during that period. We reviewed all deaths from childhood (under 15 years of age) cancers occurring in the entire state between 1944 and 1975 and assigned them to a cohort of either high or low exposure, depending on whether 15 between 1951 and 1958. For reasons unknown, leukemia mortality among the low-exposure cohort in the high-fallout counties was about half that of the United States and the remainder of the state. Mortality increased by 2.44 times (95 per cent confidence, 1.18 to 5.02) to just slightly above that of the United States in the high-exposure cohort residing in the high-fallout counties, and was greatest in 10- to 14-year-old children. For other childhood cancers, no consistent pattern was found in relation to fallout exposure. The increase in leukemia deaths could be due to fallout or to some other unexplained factor

  5. The sources and fate of radionuclides emitted to the atmosphere

    International Nuclear Information System (INIS)

    Sandalls, J.

    2001-01-01

    The thesis represents an account of the sources and fate of radionuclides entering the atmosphere, and indicates where the candidate, through his own work, has contributed to the overall picture. The sources of the natural and man-made radionuclides found in the atmosphere are identified. New data on emissions from UK coal-fired power stations and UK steel works are reported. Radionuclides produced in nuclear fission and released to the atmosphere in the detonation of nuclear weapons, in nuclear accidents, and through routine discharges from nuclear sites have added to the atmospheric burden of radioactive materials; both acute and chronic low-level emissions are discussed. The various natural processes which remove radionuclides from the atmosphere are described. Soon after release, many radioactive materials become attached to the atmospheric aerosol, but others undergo gas-phase reactions. Some gases are sufficiently long-lived in the troposphere as to find their way into the stratosphere where their fate may be determined by the short-wave radiation from the sun. The nature of the particles of fuel emitted to the atmosphere in the explosion and fire at the Chernobyl nuclear power plant in 1986 are discussed, together with the associated environmental problems. The ground is the major sink for radionuclides leaving the atmosphere, and the behaviour of the more radiologically important radionuclides following deposition is described with special reference to: (i) fallout in both the urban and living environments; (ii) the pathways which may lead to contamination of the food chain; (iii) how the fuel particle fallout from Chernobyl was unique in nuclear accidents; (iv) soil-to-plant transfer of radioelements and (v) how radiation exposure of man can be mitigated in both the contaminated urban and rural environments. (author)

  6. The partnership experience on the disposal of low- and intermediate-level short-lived waste in Belgium

    International Nuclear Information System (INIS)

    Preter, P. de; Cool, W.; Hooft, E.; Waffelaert, A.; Blommaert, J.; Draulans, J.

    2008-01-01

    With the governmental decision of January 16, 1998, the long-term storage option for the low- and intermediate-level short-lived waste (category A waste) was abandoned and ONDRAF/NIRAS was given the mission to further examine the options of deep and surface disposal, in order to prepare a federal decision on the technical option to be developed. ONDRAF/NIRAS was also asked to develop the methods and structures of interaction with the local stakeholders, and to limit its siting activities to nuclear and candidate municipalities. This brought ONDRAF/NIRAS to the concept of local partnerships with interested municipalities, and during the pre-project phase 1998-2006 partnerships were created with the municipalities of Dessel (STOLA-Dessel, 1999), Mol (MONA, 2000) and Fleurus-Farciennes (PaLoFF, 2003). On 23 June, 2006 the Belgian Government decided that category A waste will be disposed of in a near-surface repository on the territory of the Dessel municipality. This decision implies that ONDRAF/NIRAS, in further interaction with the local stakeholders, can start the preparation of a licence application. This decision was the endpoint of the pre-project phase (1998-2006) and was based on the final reports of the partnerships of Dessel (STOLA-Dessel, now STORA) and Mol (MONA), approved by their municipality councils, and on ONDRAF/NIRAS final report, confirming the feasibility of the proposed disposal systems. As the municipality council of Fleurus did not approve the final report of the partnership PaLoFF, ONDRAF/NIRAS did not submit this report to the responsible minister. The preceding positive local decision in both Dessel (May 2005) and Mol (July 2005), and both on the partnership and municipality council level, to accept, under certain conditions, a disposal facility on their territory was the result of a 6 years long process of discussions within the partnership of all aspects of the disposal system and its integration in the municipality. During these

  7. Fallout 3H ingestion in Akita, Japan

    International Nuclear Information System (INIS)

    Hisamatsu, S.; Takizawa, Y.; Abe, T.; Katsumata, T.

    1987-01-01

    To study fallout 3 H ingestion in Japan, 16 separate food group samples were collected from Akita during 1985. The 3 H concentration in free water and that in a tissue-bound form were determined separately. The average 3 H concentration in the tissue-bound form was 2.2 Bq L-1, 1.7 times higher than in the free water of the food. The ingestions of 3 H in the tissue-bound form and as free water in the diet were 0.60 Bq d-1 and 1.0 Bq d-1, respectively. Cereals represented the food group that contributed the most to the ingestion of tissue-bound 3 H. Total 3 H ingestion was estimated to be 4.1 Bq d-1. The contribution of the tissue-bound form to the total ingestion was 15%, considerably lower than reported for Italian diets. The ratio of 3 H ingestion in the tissue-bound form to the free water form in the diet was similar to the ratio reported for New York City

  8. Tracing the Iodine-129 fallout in Argentina

    Energy Technology Data Exchange (ETDEWEB)

    Fernandez Niello, Jorge; Negri, Agustin; Arazi, Andres [Comision Nacional de Energia Atomica (CNEA), Buenos Aires (Argentina). Lab. TANDAR; Wallner, Anton [The Australian National University, Canberra (Australia). Dept. of Nuclear Physics; Niello, Jorge Fernandez [Universidad Nacional de San Martin, Campus Miguelete, Buenos Aires (Argentina)

    2012-07-01

    Full text: Long-lived {sup 129}I (half-life=15.6 Ma) is produced naturally by irradiation of atmospheric xenon by cosmic neutrons and in the sub-surface by spontaneous fission of {sup 238}U, from which the natural inventory of {sup 129}I has been estimated to be around 50,000 kg, only 140 kg of them corresponds to the hydrospheric inventory. Nuclear tests and accidents have added between 45-130 kg. Apart from a global atmospheric fallout component, {sup 129}I has been released from several nuclear fuel reprocessing plants located in the Northern Hemisphere (ca. 6000 kg) which serve as localized sources in oceanographic-tracer experiments. In this presentation, we report results from a study exploring the presence of {sup 129}I in the Southern Hemisphere by determining {sup 129}I/{sup 127}I isotopic ratios in water samples (rivers, lakes and shallow sea-water) taken at different latitudes in Argentina including Antarctica. The iodine-127 and iodine-129 concentrations were measured via ICP-MS (Inductively Coupled Plasma Mass Spectrometry) and Accelerator Mass Spectrometry (AMS), respectively. Distribution of both isotopes can be understood considering tropospheric circulation patterns, possible sources and regional precipitation patterns. Natural and anthropogenic sources for the Southern Hemisphere and their inventories are discussed. Similar contribution came from natural sources and nuclear tests. Contribution from the nuclear fuel reprocessing plants placed in the Northern hemisphere can be neglected. (author)

  9. sup 111 Ag in the Chernobyl fallout

    Energy Technology Data Exchange (ETDEWEB)

    Winkler, R.; Rosner, G.; Hoetzl, H. (Gesellschaft fuer Strahlen- und Umweltforschung mbH Muenchen, Neuherberg (Germany, F.R.). Inst. fuer Strahlenschutz)

    1989-01-01

    In the course of a re-evalution of the gamma-ray spectra of air filter samples collected immediately after Chernobyl accident at Munich-Neuherberg {sup 111}Ag has been found to contribute significantly to the total activity within the first days of the Chernobyl fallout. The maximum air concentration was measured on 1 May 1986 to be 5.4 Bq/m{sup 3} compared with 9.7 Bq {sup 137}Cs per m{sup 3}. Referred to this date the total activity deposition to ground was 12{plus minus}3 kBq {sup 111}Ag per m{sup 2}. Referred to 26 April 1986 the {sup 111}Ag to {sup 110m}Ag ratio was found to be 53{plus minus}3 and the {sup 111}Ag to {sup 137}Cs ratio was 1.0{plus minus}0.1. It is estimated that the cesium isotopes were depleted during release and atmospheric transport by a factor of about 2 compared with the silver isotopes. (orig.).

  10. Health and Safety Laboratory environmental quarterly, March 1--June 1, 1976. [Fallout, natural radioactivity, and lead in environmental samples from USA, India, and Taiwan during 1976

    Energy Technology Data Exchange (ETDEWEB)

    Hardy, E.P. Jr.

    1976-07-01

    This report presents current data from the HASL environmental programs, the Air Monitoring Section of the Bhabha Atomic Research Center in India, the Health Physics Section of the Institute of Nuclear Science in Taiwan and the Radiological and Environmental Research Division at Argonne National Laboratory. The initial section consists of interpretive reports and notes on the history of long-range fallout, cesium-137 in Bombay milk, natural and fallout radioactivity in Indian diet, reporting results of radioactivity measurements at near zero levels of sample activity and background, plutonium in soil northeast of the Nevada Test Site, radon levels at the Lloyd, NY regional station, strontium-90 in New York and San Francisco diets through 1975, plutonium-239, 240 in 1974 diet, up-dating stratospheric radionuclide inventories to July 1975 and a revised table of radionuclides. Subsequent sections include tabulations of radionuclide levels in stratospheric air; lead and radionuclides in surface air; strontium-90 in deposition, milk, diet, tap water, and human bone; cesium-137 in Chicago foods in April 1976; and environmental radioactivity surveys for nuclear power plants in North Taiwan. A bibliography of recent publications related to environmental studies is also presented.

  11. The transport of fallout 137Cs within undisturbed soils in Nigeria based on measured soil concentration profiles

    International Nuclear Information System (INIS)

    Ajayi, I.R.

    2007-12-01

    The transport of fallout 137 Cs within the Nigerian soil has been studied in this paper by the compartment and the diffusion-convection models. The measured concentrations of the radionuclide in the soil layers were examined by the models in order to estimate the transport parameters of residence half-time, migration velocity, diffusion coefficient and the convective velocities of the radionuclide within the soils. The residence half-times were observed to be short and decreased with soil depth with a mean ranging from 0.3 years at 0 - 2cm soil depth in the Akure site to 1.4 years at 10-15cm depth in the Igbeti site. The migration velocity ν, calculated from the residence times with the consideration of the different thicknesses of layers were observed to decrease slowly with depth at all the sampling sites with a range from 3.62 cm y -1 at the Igbeti site to 8.21 cm.y -1 at the Ikogosi site. The migration velocities obtained are quite higher than those reported in literature for global fallout. The range of the diffusion coefficient was 0.72 - 1.02 cm 2 per year while that of the convective velocity was from 0.07 to 0.16 cm per year. Diffusion coefficients were observed to be higher than the convective velocities at all sampling points. (author)

  12. Tracing the Chernobyl fall-out peak in Finnish lake sediments in order to obtain a good time marker

    International Nuclear Information System (INIS)

    Jungner, H.

    1998-01-01

    The fall-out 137 Cs from the Chernobyl accident has been traced in sediments from a few lakes in Finland in order to obtain a time marker in the uppermost sediment layer. A beta multicounter system developed at Risoe was used for detection of the radionuclides. The detector system is based on GM counters and has therefore no energy resolution. It is thus not possible to identify different nuclides with the counting system. The low background and good efficiency of this detector makes it possible to use small amount of sample and thus good depth resolution can be obtained for the sediment profile. A clear advantage is that practically no sample preparation is needed. Beside providing a time marker for year 1986 in a sediment, the activity depth profile obtained can provide information about sedimentation conditions and the removal of the fall-out cesium from the lake water. The influence from natural radionuclides in the sediment material, however, puts a limit to the lowest detection level, and makes detailed mobility studies difficult. For direct home marking the beta counter is, however, an effective tool. (orig.)

  13. Cesium, iodine and tritium in NW Pacific waters – a comparison of the Fukushima impact with global fallout

    Directory of Open Access Journals (Sweden)

    P. P. Povinec

    2013-08-01

    Full Text Available Radionuclide impact of the Fukushima Dai-ichi nuclear power plant accident on the distribution of radionuclides in seawater of the NW Pacific Ocean is compared with global fallout from atmospheric tests of nuclear weapons. Surface and water column samples collected during the Ka'imikai-o-Kanaloa (KOK international expedition carried out in June 2011 were analyzed for 134Cs, 137Cs, 129I and 3H. The 137Cs, 129I and 3H levels in surface seawater offshore Fukushima varied between 0.002–3.5 Bq L−1, 0.01–0.8 μBq L−1, and 0.05–0.15 Bq L−1, respectively. At the sampling site about 40 km from the coast, where all three radionuclides were analyzed, the Fukushima impact on the levels of these three radionuclides represents an increase above the global fallout background by factors of about 1000, 50 and 3, respectively. The water column data indicate that the transport of Fukushima-derived radionuclides downward to the depth of 300 m has already occurred. The observed 137Cs levels in surface waters and in the water column are compared with predictions obtained from the ocean general circulation model, which indicates that the Kuroshio Current acts as a southern boundary for the transport of the radionuclides, which have been transported from the Fukushima coast eastward in the NW Pacific Ocean. The 137Cs inventory in the water column is estimated to be about 2.2 PBq, what can be regarded as a lower limit of the direct liquid discharges into the sea as the seawater sampling was carried out only in the area from 34 to 37° N, and from 142 to 147° E. About 4.6 GBq of 129I was deposited in the NW Pacific Ocean, and 2.4–7 GBq of 129I was directly discharged as liquid wastes into the sea offshore Fukushima. The total amount of 3H released and deposited over the NW Pacific Ocean was estimated to be 0.1–0.5 PBq. These estimations depend, however, on the evaluation of the total 137Cs activities released as liquid wastes directly into the sea, which

  14. Cesium, iodine and tritium in NW Pacific waters - a comparison of the Fukushima impact with global fallout

    Science.gov (United States)

    Povinec, P. P.; Aoyama, M.; Biddulph, D.; Breier, R.; Buesseler, K.; Chang, C. C.; Golser, R.; Hou, X. L.; Ješkovský, M.; Jull, A. J. T.; Kaizer, J.; Nakano, M.; Nies, H.; Palcsu, L.; Papp, L.; Pham, M. K.; Steier, P.; Zhang, L. Y.

    2013-08-01

    Radionuclide impact of the Fukushima Dai-ichi nuclear power plant accident on the distribution of radionuclides in seawater of the NW Pacific Ocean is compared with global fallout from atmospheric tests of nuclear weapons. Surface and water column samples collected during the Ka'imikai-o-Kanaloa (KOK) international expedition carried out in June 2011 were analyzed for 134Cs, 137Cs, 129I and 3H. The 137Cs, 129I and 3H levels in surface seawater offshore Fukushima varied between 0.002-3.5 Bq L-1, 0.01-0.8 μBq L-1, and 0.05-0.15 Bq L-1, respectively. At the sampling site about 40 km from the coast, where all three radionuclides were analyzed, the Fukushima impact on the levels of these three radionuclides represents an increase above the global fallout background by factors of about 1000, 50 and 3, respectively. The water column data indicate that the transport of Fukushima-derived radionuclides downward to the depth of 300 m has already occurred. The observed 137Cs levels in surface waters and in the water column are compared with predictions obtained from the ocean general circulation model, which indicates that the Kuroshio Current acts as a southern boundary for the transport of the radionuclides, which have been transported from the Fukushima coast eastward in the NW Pacific Ocean. The 137Cs inventory in the water column is estimated to be about 2.2 PBq, what can be regarded as a lower limit of the direct liquid discharges into the sea as the seawater sampling was carried out only in the area from 34 to 37° N, and from 142 to 147° E. About 4.6 GBq of 129I was deposited in the NW Pacific Ocean, and 2.4-7 GBq of 129I was directly discharged as liquid wastes into the sea offshore Fukushima. The total amount of 3H released and deposited over the NW Pacific Ocean was estimated to be 0.1-0.5 PBq. These estimations depend, however, on the evaluation of the total 137Cs activities released as liquid wastes directly into the sea, which should improve when more data are

  15. Decontamination of radionuclides in food

    Energy Technology Data Exchange (ETDEWEB)

    Ohmomo, Yoichiro [Institute for Environmental Sciences, Aomori (Japan)

    1994-03-01

    The release of radionuclides arising from the Chernobyle accident led to widespread contamination of the northern hemisphere through fallout. This accident provided again an opportunity to investigate how and to what extent the radionuclides contamination in crops and animal derived foods could be reduced. The following topics are included in this paper. (1) How to reduce the transfer of radiostrontium and/or cesium from soil to crops: A pH increase of soil is effective for reducing their plant uptake. (2) How to reduce the transfer of radiocesium to animal derived foods: Ammonium-ferric-cyanoferrate (AFCF) should be the most effective compound for radiocesium excretion in the feces. Experiments with lactating cows and/or poultry gave extremely good results with respect to low radiocesium concentrations in milk, meat and eggs. (3) Removal coefficients of radiostrontium, cesium and iodine from contaminated leaf vegetables and cereals during food processing and culinary preparation: Though different by species, more than 80% of cesium and about 50% of strontium and iodine can be removed during culinary preparation of washing and boiling. (4) Simultaneous decontamination of radiocesium and iodine from drinking water and liquid milk: Metal ferrocyanide-anion exchange resin, specifically Fe ferrocyanide one, was successfully used for a rapid and simple decontamination of radiocesium and iodine in the liquid samples arising from the Chernobyle accident. (5) Removal of radiocesium from meat: The meat structurally contaminated with radiocesium is easily and very successfully decontaminated by pickling in NaCl solution and the decontamination is much speeded up by freezing meat before pickling. (author).

  16. Decontamination of radionuclides in food

    International Nuclear Information System (INIS)

    Ohmomo, Yoichiro

    1994-01-01

    The release of radionuclides arising from the Chernobyle accident led to widespread contamination of the northern hemisphere through fallout. This accident provided again an opportunity to investigate how and to what extent the radionuclides contamination in crops and animal derived foods could be reduced. The following topics are included in this paper. (1) How to reduce the transfer of radiostrontium and/or cesium from soil to crops: A pH increase of soil is effective for reducing their plant uptake. (2) How to reduce the transfer of radiocesium to animal derived foods: Ammonium-ferric-cyanoferrate (AFCF) should be the most effective compound for radiocesium excretion in the feces. Experiments with lactating cows and/or poultry gave extremely good results with respect to low radiocesium concentrations in milk, meat and eggs. (3) Removal coefficients of radiostrontium, cesium and iodine from contaminated leaf vegetables and cereals during food processing and culinary preparation: Though different by species, more than 80% of cesium and about 50% of strontium and iodine can be removed during culinary preparation of washing and boiling. (4) Simultaneous decontamination of radiocesium and iodine from drinking water and liquid milk: Metal ferrocyanide-anion exchange resin, specifically Fe ferrocyanide one, was successfully used for a rapid and simple decontamination of radiocesium and iodine in the liquid samples arising from the Chernobyle accident. (5) Removal of radiocesium from meat: The meat structurally contaminated with radiocesium is easily and very successfully decontaminated by pickling in NaCl solution and the decontamination is much speeded up by freezing meat before pickling. (author)

  17. A MODEL BUILDING CODE ARTICLE ON FALLOUT SHELTERS WITH RECOMMENDATIONS FOR INCLUSION OF REQUIREMENTS FOR FALLOUT SHELTER CONSTRUCTION IN FOUR NATIONAL MODEL BUILDING CODES.

    Science.gov (United States)

    American Inst. of Architects, Washington, DC.

    A MODEL BUILDING CODE FOR FALLOUT SHELTERS WAS DRAWN UP FOR INCLUSION IN FOUR NATIONAL MODEL BUILDING CODES. DISCUSSION IS GIVEN OF FALLOUT SHELTERS WITH RESPECT TO--(1) NUCLEAR RADIATION, (2) NATIONAL POLICIES, AND (3) COMMUNITY PLANNING. FALLOUT SHELTER REQUIREMENTS FOR SHIELDING, SPACE, VENTILATION, CONSTRUCTION, AND SERVICES SUCH AS ELECTRICAL…

  18. Nuclear physics with use of KUR. Reviews of 30 years studies on short-lived nuclei and perspectives for the future

    International Nuclear Information System (INIS)

    Kawase, Yoichi

    1995-01-01

    The research works which were carried out over the past 30 years on nuclear structure study have been reviewed with emphasis on the technical developments of experimental apparatus for the studies of very short-lived isotopes produced by the Kyoto University reactor(KUR). In the first chapter, nuclear structure studies of neutron-rich nuclei with use of the on-line irradiation apparatus and the on-line isotope separator(ISOL) for fission products have been described. In the second chapter, applications of nuclear methods to solid state physics by the perturbed angular correlation(PAC) technique have been examined to investigate the local electromagnetic fields in metals and compounds through the hyperfine interactions. Perspectives for the future of related research fields are given aiming at the advanced uses of short-lived radioisotopes. (author)

  19. Radionuclide Basics: Technetium-99

    Science.gov (United States)

    Technetium-99 (chemical symbol Tc-99) is a silver-gray, radioactive metal. It occurs naturally in very small amounts in the earth's crust, but is primarily man-made. Technetium-99m is a short-lived form of Tc-99 that is used as a medical diagnostic tool.

  20. Radionuclide transfer from soil to plants

    International Nuclear Information System (INIS)

    Teufel, D.; Steinhilber-Schwab, B.; Hoepfner, U.; Ratka, R.; Sand, H. van de; Franke, B.

    1979-01-01

    The planned nuclear reprocessing plant (NEZ) Gorleben will fundamentally differ from actually operating nuclear power plants with regard to its radioactive emissions because relatively long-life isotopes will play a greater role in the emissions. The longevity of the radionuclides emitted in the planned NEZ implies that there will be an accumulation of radionuclides in the surroundings of the plant and long-term effects of the plant on the environment will get higher significance. As radionuclides mainly reach milk and meat via the food of farm animals the transfer of cesium and strontium from the ground into plants was amply investigated. The results show that the correlation calculations are suitable to describe the effect of different parameters on the transfer factor. They are not suited for a forecast of the transfer conditions on a certain location for the reasons explained before. Location-specific measurements seem to be indispensable for these purposes. Besides the greenhouse tests open air measurements of fall-out nuclides with and without elimination of external contamination seem to represent a realistic possibility for the determination of transfer factors. Great attention has to be paid in this kind of tests to the growth conditions (especially fertilization) which have to be accurately registered. (orig./MG) [de