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Sample records for resonant magnetic x-ray

  1. Resonance magnetic x-ray scattering study of erbium

    DEFF Research Database (Denmark)

    Sanyal, M.K.; Gibbs, D.; Bohr, J.

    1994-01-01

    The magnetic phases of erbium have been studied by resonance x-ray-scattering techniques. When the incident x-ray energy is tuned near the L(III) absorption edge, large resonant enhancements of the magnetic scattering are observed above 18 K. We have measured the energy and polarization dependence...... of this magnetic scattering and analyzed it using a simple model based on electric dipole and quadrupole transitions among atomic orbitals. The line shapes can be fitted to a magnetic structure combining both c-axis-modulated and basal-plane components. Below 18 K, we have observed unusual behavior of the magnetic...... scattering as a function of energy, whose origin is not understood....

  2. Resonant magnetic scattering of polarized soft x rays

    Energy Technology Data Exchange (ETDEWEB)

    Sacchi, M. [Centre Universitaire Paris-Sud, Orsay (France); Hague, C.F. [Universite Pierre et Marie Curie, Paris (France); Gullikson, E.M.; Underwood, J. [Ernest Orlando Lawrence Berkeley National Lab., CA (United States)

    1997-04-01

    Magnetic effects on X-ray scattering (Bragg diffraction, specular reflectivity or diffuse scattering) are a well known phenomenon, and they also represent a powerful tool for investigating magnetic materials since it was shown that they are strongly enhanced when the photon energy is tuned across an absorption edge (resonant process). The resonant enhancement of the magnetic scattering has mainly been investigated at high photon energies, in order to match the Bragg law for the typical lattice spacings of crystals. In the soft X-ray range, even larger effects are expected, working for instance at the 2p edges of transition metals of the first row or at the 3d edges of rare earths (300-1500 eV), but the corresponding long wavelengths prevent the use of single crystals. Two approaches have been recently adopted in this energy range: (i) the study of the Bragg diffraction from artificial structures of appropriate 2d spacing; (ii) the analysis of the specular reflectivity, which contains analogous information but has no constraints related to the lattice spacing. Both approaches have their own specific advantages: for instance, working under Bragg conditions provides information about the (magnetic) periodicity in ordered structures, while resonant reflectivity can easily be related to electronic properties and absorption spectra. An important aspect common to all the resonant X-ray scattering techniques is the element selectivity inherent to the fact of working at a specific absorption edge: under these conditions, X-ray scattering becomes in fact a spectroscopy. Results are presented for films of iron and cobalt.

  3. Magnetic resonance imaging of the central nervous system. Comparison with X-ray CT

    Energy Technology Data Exchange (ETDEWEB)

    Kajima, Toshio; Kagawa, Yoshihiro; Katsuta, Shizutomo.

    1987-06-01

    Magnetic resonance imaging (MRI) and X-ray computed tomography (X-ray CT) have been performed in 169 consecutive patients with central nervous system diseases. The findings from the two methods were compared for the capacity to defect lesions. Magnetic resonance imaging was more sensitive than or equivalent to X-ray CT in detecting lesions - especially detecting. Arnold-Chiari malformation, syringomyelia, spinal cord injury, and pituitary adenoma - in 158 patients (94 %). In six patients (10 %), lesion detection was possible only by MRI. Magnetic resonance imaging was inferior to X-ray CT in 11 patients (7 %) in detecting calcified lesions, meningioma, and cavernous hemangioma. (Namekawa, K.).

  4. Magnetism in heterogeneous thin film systems: Resonant x-ray scattering studies

    Energy Technology Data Exchange (ETDEWEB)

    Kortright, J.B.; Jiang, J.S.; Bader, S.D.; Hellwig, O.; Marguiles, D.T.; Fullerton, E.E.

    2002-10-28

    Magnetic and chemical heterogeneity are common in a broad range of magnetic thin film systems. Emerging resonant soft x-ray scattering techniques are well suited to resolve such heterogeneity at relevant length scales. Resonant x-ray magneto-optical Kerr effect measurements laterally average over heterogeneity but can provide depth resolution in different ways, as illustrated in measurements resolving reversible and irreversible changes in different layers of exchange-spring heterostructures. Resonant small-angle scattering measures in-plane heterogeneity and can resolve magnetic and chemical scattering sources in different ways, as illustrated in measurements of granular alloy recording media.

  5. Magnetic x-ray linear dichroism in resonant and non-resonant Gd 4f photoemission

    Energy Technology Data Exchange (ETDEWEB)

    Mishra, S.; Gammon, W.J.; Pappas, D.P. [Virginia Commonwealth Univ., Richmond, VA (United States)] [and others

    1997-04-01

    The enhancement of the magnetic linear dichroism in resonant 4f photoemission (MLDRPE) is studied from a 50 monolayer film of Gd/Y(0001). The ALS at beamline 7.0.1 provided the source of linearly polarized x-rays used in this study. The polarized light was incident at an angle of 30 degrees relative to the film plane, and the sample magnetization was perpendicular to the photon polarization. The linear dichroism of the 4f core levels is measured as the photon energy is tuned through the 4d-4f resonance. The authors find that the MLDRPE asymmetry is strongest at the resonance. Near the threshold the asymmetry has several features which are out of phase with the fine structure of the total yield.

  6. ALICE: A diffractometer/reflectometer for soft X-ray resonant magnetic scattering at BESSY II

    Directory of Open Access Journals (Sweden)

    Radu-Marius Abrudan

    2016-05-01

    Full Text Available Although the chamber named ALICE was designed for the analysis of magnetic hetero- and nanostructures via resonant magnetic x-ray scattering, the instrument is not limited to this technique. Static measurements involve the possibility to use scattering and spectroscopy synchrotron based techniques (photon-in photon-out, photon-in electron-out, and coherent scattering. Dynamic experiments require either laser or magnetic field pulses to excite the spin system followed by x-ray probe in the time domain from nano- to femtosecond delay times. In this temporal range, the demagnetization/remagnetization dynamics and magnetization precession in a number of magnetic materials (metals, alloys, and magnetic multilayers can be probed in an element specific manner. The versatility of the instrument was tested by a series of pilot experiments, pointing out ALICE as one of the most demanded instruments at the Helmholtz-Zentrum in Berlin.

  7. Magnetic hysteresis of an artificial square ice studied by in-plane Bragg x-ray resonant magnetic scattering

    Directory of Open Access Journals (Sweden)

    J. P. Morgan

    2012-06-01

    Full Text Available We report X-ray resonant magnetic scattering studies of a Permalloy artificial square ice nanomagnet array, focussing on the field-driven evolution of the sum Σ and difference Δ signals of left and right handed circularly polarized synchrotron X-rays at different lateral positions in reciprocal space Qx. We used X-rays tuned to the Fe L3 resonance energy, with the scattering plane aligned along a principal symmetry axis of the array. Details of the specular Δ hysteresis curve are discussed, following the system magnetization from an initial demagnetized state. The periodic structure gives rise to distinct peaks at in-plane reciprocal Bragg positions, as shown by fitting Σ(Qx to a model based on a simple unit cell structure. Diffraction order-dependent hysteresis in Δ is observed, indicative of the reordering of magnetization on the system's two interpenetrating sublattices, which markedly deviates from an ideal Ising picture under strong applied fields.

  8. Non-resonant magnetic X-ray scattering on NdCu 2

    Science.gov (United States)

    Schneidewind, A.; Loewenhaupt, M.; Hiess, A.; Kramp, S.; Reif, T.; Neubeck, W.; Vettier, C.

    2001-07-01

    The zero-field magnetic phases of NdCu 2 have been investigated using non-resonant X-ray scattering and the results are compared to those from neutron scattering. The reduced scattering volume of X-ray scattering as opposed to the bulk average measured by neutron scattering allowed us to investigate the magnetic properties in the near-surface region. As in the neutron scattering experiment, three magnetic phases AF1, AF2 and AF3 have been observed, and they exist in the same degree of order as the crystal lattice. In the near-surface region, the large magnetic unit cell present in AF2 is slightly different as compared to the bulk. Our results validate the first order of the phase transitions between the magnetic phases and allow us to localize the stabilization of the magnetic phase AF2 in real space. The modulation of the low-temperature structures AF1 and AF2 are squared up. In addition, we find a magnetically induced modulation of the electronic distribution in the low-temperature phase AF1 which is consistent with a lattice distortion (magneto-elastic coupling).

  9. Non-resonant magnetic X-ray scattering on NdCu{sub 2}

    Energy Technology Data Exchange (ETDEWEB)

    Schneidewind, A.; Loewenhaupt, M. E-mail: loewenhaupt@physik.tu-dresden.de; Hiess, A.; Kramp, S.; Reif, T.; Neubeck, W.; Vettier, C

    2001-07-01

    The zero-field magnetic phases of NdCu{sub 2} have been investigated using non-resonant X-ray scattering and the results are compared to those from neutron scattering. The reduced scattering volume of X-ray scattering as opposed to the bulk average measured by neutron scattering allowed us to investigate the magnetic properties in the near-surface region. As in the neutron scattering experiment, three magnetic phases AF1, AF2 and AF3 have been observed, and they exist in the same degree of order as the crystal lattice. In the near-surface region, the large magnetic unit cell present in AF2 is slightly different as compared to the bulk. Our results validate the first order of the phase transitions between the magnetic phases and allow us to localize the stabilization of the magnetic phase AF2 in real space. The modulation of the low-temperature structures AF1 and AF2 are squared up. In addition, we find a magnetically induced modulation of the electronic distribution in the low-temperature phase AF1 which is consistent with a lattice distortion (magneto-elastic coupling)

  10. Soft x-ray resonant diffraction study of magnetic and orbital correlations in a manganite near half doping

    NARCIS (Netherlands)

    Thomas, KJ; Grenier, S; Kim, YJ; Abbamonte, P; Rusydi, A; Tomioka, Y; Tokura, Y; McMorrow, DF; Sawatzky, G; van Veenendaal, M; Hill, J.P.; Venema, L.C.

    2004-01-01

    We have utilized resonant x-ray diffraction at the Mn L(II,III) edges in order to directly compare magnetic and orbital correlations in Pr(0.6)Ca(0.4)MnO(3). Comparing the widths of the magnetic and orbital diffraction peaks, we find that the magnetic correlation length exceeds that of the orbital o

  11. Interplay between structure and magnetism in HoxPr1-x alloys. 2. Resonant x-ray magnetic scattering

    DEFF Research Database (Denmark)

    Vigliante, A.; Christensen, M.J.; Hill, J.P.;

    1998-01-01

    X-ray-scattering techniques have been used to study the crystal and magnetic structures of HoxPr1-x alloys in the form of thin films. Three distinct crystal structures are found as a function of concentration x, each of which has a characteristic magnetic structure. For x greater than or equal to 0.......6 a hexagonal-close-packed phase is found with the magnetic moments ordered in a basal-plane helix, whereas for 0.4 less than or equal to x... hexagonal-close-packed and remain nonmagnetic down to the lowest temperatures studied. Using x-ray magnetic resonance scattering techniques, we demonstrate that a small, static spin-density wave is induced within the alloy 5d band at both the Pr and Ho sites in both of the magnetically ordered phases...

  12. A complete software application for automatic registration of x-ray mammography and magnetic resonance images

    Energy Technology Data Exchange (ETDEWEB)

    Solves-Llorens, J. A.; Rupérez, M. J., E-mail: mjruperez@labhuman.i3bh.es; Monserrat, C. [LabHuman, Universitat Politècnica de València, Camino de Vera s/n, 46022 Valencia (Spain); Feliu, E.; García, M. [Hospital Clínica Benidorm, Avda. Alfonso Puchades, 8, 03501 Benidorm (Alicante) (Spain); Lloret, M. [Hospital Universitari y Politècnic La Fe, Bulevar Sur, 46026 Valencia (Spain)

    2014-08-15

    Purpose: This work presents a complete and automatic software application to aid radiologists in breast cancer diagnosis. The application is a fully automated method that performs a complete registration of magnetic resonance (MR) images and x-ray (XR) images in both directions (from MR to XR and from XR to MR) and for both x-ray mammograms, craniocaudal (CC), and mediolateral oblique (MLO). This new approximation allows radiologists to mark points in the MR images and, without any manual intervention, it provides their corresponding points in both types of XR mammograms and vice versa. Methods: The application automatically segments magnetic resonance images and x-ray images using the C-Means method and the Otsu method, respectively. It compresses the magnetic resonance images in both directions, CC and MLO, using a biomechanical model of the breast that distinguishes the specific biomechanical behavior of each one of its three tissues (skin, fat, and glandular tissue) separately. It makes a projection of both compressions and registers them with the original XR images using affine transformations and nonrigid registration methods. Results: The application has been validated by two expert radiologists. This was carried out through a quantitative validation on 14 data sets in which the Euclidean distance between points marked by the radiologists and the corresponding points obtained by the application were measured. The results showed a mean error of 4.2 ± 1.9 mm for the MRI to CC registration, 4.8 ± 1.3 mm for the MRI to MLO registration, and 4.1 ± 1.3 mm for the CC and MLO to MRI registration. Conclusions: A complete software application that automatically registers XR and MR images of the breast has been implemented. The application permits radiologists to estimate the position of a lesion that is suspected of being a tumor in an imaging modality based on its position in another different modality with a clinically acceptable error. The results show that the

  13. A compact permanent-magnet system for measuring magnetic circular dichroism in resonant inelastic soft X-ray scattering.

    Science.gov (United States)

    Miyawaki, Jun; Suga, Shigemasa; Fujiwara, Hidenori; Niwa, Hideharu; Kiuchi, Hisao; Harada, Yoshihisa

    2017-03-01

    A compact and portable magnet system for measuring magnetic dichroism in resonant inelastic soft X-ray scattering (SX-RIXS) has been developed at the beamline BL07LSU in SPring-8. A magnetic circuit composed of Nd-Fe-B permanent magnets, which realised ∼0.25 T at the center of an 11 mm gap, was rotatable around the axis perpendicular to the X-ray scattering plane. Using the system, a SX-RIXS spectrum was obtained under the application of the magnetic field at an angle parallel, nearly 45° or perpendicular to the incident X-rays. A dedicated sample stage was also designed to be as compact as possible, making it possible to perform SX-RIXS measurements at arbitrary incident angles by rotating the sample stage in the gap between the magnetic poles. This system enables facile studies of magnetic dichroism in SX-RIXS for various experimental geometries of the sample and the magnetic field. A brief demonstration of the application is presented.

  14. Gorham disease of the craniocervical junction: X-ray, computed tomography, and magnetic resonance imaging findings.

    Science.gov (United States)

    Kilicoglu, Z Gamze; Kizildemir Kis, Naciye; Vardar Aker, Fügen; Berkman, M Zafer; Simsek, M Masum

    2013-05-01

    Gorham disease of massive osteolysis is a spontaneous, idiopathic, and progressive form of primary osteolysis. It has no age, sex, or race predilection, and patients are mostly asymptomatic until severe deformity or pathological fracture becomes evident. A patient with craniocervical involvement is presented, describing imaging findings with a review of the literature to provide an insight into the disorder. Case report and review of the literature. X-ray, computed tomography, and magnetic resonance imaging findings of a patient with findings related to the site of involvement. All images demonstrate osteolysis typically described for the disease. Differential diagnosis and key features are indicated. Operative findings and pathological analysis were also consistent with the findings. Patient's follow-up is also reported. This benign appearing yet disabling disease may become fatal in relation to the site involved. Acknowledging imaging findings may provide early diagnosis for timely intervention or supportive management. Copyright © 2013 Elsevier Inc. All rights reserved.

  15. Dynamical process of skyrmion-helical magnetic transformation of the chiral-lattice magnet FeGe probed by small-angle resonant soft x-ray scattering

    Science.gov (United States)

    Yamasaki, Y.; Morikawa, D.; Honda, T.; Nakao, H.; Murakami, Y.; Kanazawa, N.; Kawasaki, M.; Arima, T.; Tokura, Y.

    2015-12-01

    Small-angle soft x-ray scattering in resonance with Fe L absorption edge has been investigated for helical magnetic order and magnetic skyrmion crystal (SkX) in B20-type cubic FeGe. Transformation of magnetic structures among helical, conical, SkX, and field-polarized spin-collinear forms is observed with the application of a magnetic field parallel to the incident soft x-ray. The resonant soft x-ray scattering with high q -resolution revealed a transient dynamics of SkX, such as rotation of SkX and variation of the SkX lattice constant, upon the change of magnetic field.

  16. Perpendicular magnetic anisotropy in ultrathin Co|Ni multilayer films studied with ferromagnetic resonance and magnetic x-ray microspectroscopy

    Energy Technology Data Exchange (ETDEWEB)

    Macia, F., E-mail: ferran.macia@gmail.com [Department of Physics, New York University, 4 Washington Place, New York, NY 10003 (United States); Warnicke, P. [National Synchrotron Light Source, Brookhaven National Laboratory, Upton, NY 11973 (United States); Bedau, D. [Department of Physics, New York University, 4 Washington Place, New York, NY 10003 (United States); Im, M.-Y.; Fischer, P. [Center for X-ray Optics, Lawrence Berkeley National Laboratory, Berkeley, CA 94720 (United States); Arena, D.A. [National Synchrotron Light Source, Brookhaven National Laboratory, Upton, NY 11973 (United States); Kent, A.D. [Department of Physics, New York University, 4 Washington Place, New York, NY 10003 (United States)

    2012-11-15

    Ferromagnetic resonance (FMR) spectroscopy, x-ray magnetic circular dichroism (XMCD) spectroscopy and magnetic transmission soft x-ray microscopy (MTXM) experiments have been performed to gain insight into the magnetic anisotropy and domain structure of ultrathin Co|Ni multilayer films with a thin permalloy layer underneath. MTXM images with a spatial resolution better than 25 nm were obtained at the Co L{sub 3} edge down to an equivalent thickness of Co of only 1 nm, which establishes a new lower boundary on the sensitivity limit of MTXM. Domain sizes are shown to be strong functions of the anisotropy and thickness of the film. - Highlights: Black-Right-Pointing-Pointer We show record sensitivity of x-ray microscopy in a 1 nm Co effective thickness. Black-Right-Pointing-Pointer We found extreme sensitivity of the domain structure to number of bilayer repeats. Black-Right-Pointing-Pointer Perpendicular anisotropy is nearly independent of the number of bilayers. Black-Right-Pointing-Pointer We have combined Ferromagnetic resonance and high resolution XMCD microscopy.

  17. K-edge resonant x-ray magnetic scattering from a transition-metal oxide: NiO

    DEFF Research Database (Denmark)

    Hill, J.P.; Kao, C.C.; McMorrow, D.F.

    1997-01-01

    We report the observation of resonant x-ray magnetic scattering in the vicinity of the Ni K edge in the antiferromagnet NiO. An approximately twofold increase in the scattering is observed as the incident photon energy is tuned through a pre-edge feature in the absorption spectrum, associated...

  18. Magnetic Resonance Urography and X-ray Urography Findings of Congenital Megaureter

    Institute of Scientific and Technical Information of China (English)

    Tian-ran Li; Xiang-ke Du; Tian-Iong Huo

    2011-01-01

    Objective To observe the imaging findings of congenital megaureter in order to enhance the understanding of this disease.Methods Image data of 5 patients with congenital megaureter and 2 misdiagnosed patients were analyzed, and image findings of congenital megaureter were summarized. Elscint Prestig 2.0T superconductive magnetic resonance urography (MRU) with conventional sequence (spin-echo, T1WI 560 ms/16 ms; fast spin-echo, T2WI 9600 ms/96 ms) was performed. Raw data were acquired with fast spin-echo sequence from heavy T2-weighted image (9600 ms/120 ms). Post-processing method of MRU was the maximum intensity projection with three-dimensional reconstruction in the workstation. Intravenous pyelography (IVP) was conducted, in which X-ray films were taken 7 minutes, 15 minutes, and 30 minutes after injecting contrast agent, except that in 2 patients the films were taken delayed at 60 and 90 minutes. X-ray retrograde pyelography was performed on 2 patients, successful in one but failed in the other. Results The dilated ureter showed hypointensity on T1-weighted images and hyperintensity on T2-weighted images in conventional MRI. The mass wall was intact, uniform in thickness, and showing hypointensity on T1-weighted and T2-weighted images. The MRH images showed a retroperitoneal mass appearing as an elongated tubular cystic structure spreading from kidney to bladder. MRH also revealed dilated calices and renal pelvis, pelviureteric obstruction, and renal duplication. The main signs of congenital megaureter in X-urography was significant dilatation of ureter, or normal renal pelvis with ureter dilatation,hydronephrosis, deformity, and displacement.Conclusions MRU with X-urography could visualize the characteristics of congenital megaureter, including the dilation of renal pelvis and ureter, calculi, urinary tract duplication, and stenosis location. The two techniques can complement each other in disease diagnosis and provide more detailed information for

  19. Theoretical approach to direct resonant inelastic X-ray scattering on magnets and superconductors

    Energy Technology Data Exchange (ETDEWEB)

    Marra, Pasquale

    2015-10-26

    The capability to probe the dispersion of elementary spin, charge, orbital, and lattice excitations has positioned resonant inelastic X-ray scattering (RIXS) at the forefront of photon science. In this work, we will investigate how RIXS can contribute to a deeper understanding of the orbital properties and of the pairing mechanism in unconventional high-temperature superconductors. In particular, we show how direct RIXS spectra of magnetic excitations can reveal long-range orbital correlations in transition metal compounds, by discriminating different kind of orbital order in magnetic and antiferromagnetic systems. Moreover, we show how RIXS spectra of quasiparticle excitations in superconductors can measure the superconducting gap magnitude, and reveal the presence of nodal points and phase differences of the superconducting order parameter on the Fermi surface. This can reveal the properties of the underlying pairing mechanism in unconventional superconductors, in particular cuprates and iron pnictides, discriminating between different superconducting order parameter symmetries, such as s,d (singlet pairing) and p wave (triplet pairing).

  20. Quantitative Imaging of Cell-Permeable Magnetic Resonance Contrast Agents Using X-Ray Fluorescence

    Directory of Open Access Journals (Sweden)

    Paul J. Endres

    2006-10-01

    Full Text Available The inability to transduce cellular membranes is a limitation of current magnetic resonance imaging probes used in biologic and clinical settings. This constraint confines contrast agents to extracellular and vascular regions of the body, drastically reducing their viability for investigating processes and cycles in developmental biology. Conversely, a contrast agent with the ability to permeate cell membranes could be used in visualizing cell patterning, cell fate mapping, gene therapy, and, eventually, noninvasive cancer diagnosis. Therefore, we describe the synthesis and quantitative imaging of four contrast agents with the capability to cross cell membranes in sufficient quantity for detection. Each agent is based on the conjugation of a Gd(III chelator with a cellular transduction moiety. Specifically, we coupled Gd(III–diethylenetriaminepentaacetic acid DTPA and Gd(III–1,4,7,10-tetraazacyclododecane-1,4,7,10-tetraacetic acid with an 8–amino acid polyarginine oligomer and an amphipathic stilbene molecule, 4-amino-4'-(N,N-dimethylaminostilbene. The imaging modality that provided the best sensitivity and spatial resolution for direct detection of the contrast agents is synchrotron radiation x-ray fluorescence (SR-XRF. Unlike optical microscopy, SR-XRF provides two-dimensional images with resolution 103 better than 153Gd gamma counting, without altering the agent by organic fluorophore conjugation. The transduction efficiency of the intracellular agents was evaluated by T1 analysis and inductively coupled plasma mass spectrometry to determine the efficacy of each chelate-transporter combination.

  1. [Characterization of biochar by X-ray photoelectron spectroscopy and 13C nuclear magnetic resonance].

    Science.gov (United States)

    Xu, Dong-yu; Jin, Jie; Yan, Yu; Han, Lan-fang; Kang, Ming-jie; Wang, Zi-ying; Zhao, Ye; Sun, Ke

    2014-12-01

    The wood (willow branch) and grass (rice straw) materials were pyrolyzed at different temperatures (300, 450 and 600 °C) to obtain the biochars used in the present study. The biochars were characterized using elementary analysis, X-ray photoelectron spectroscopy (XPS) and solid state 13C cross-polarization and magic angle spinning nuclear magnetic resonance spectroscopy (13C NMR) to illuminate the structure and composition of the biochars which were derived from the different thermal temperatures and biomass. The results showed that the H/C, O/C and (O+N)/C ratios of the biochars decreased with the increase in the pyrolysis temperatures. The surface polarity and ash content of the grass-derived biochars were higher than those of the wood-derived biochars. The minerals of the wood-derived biochars were mainly covered by the organic matter; in contrast, parts of the mineral surfaces of the grass-derived biochars were not covered by organic matter? The 13C NMR of the low temperature-derived biochars revealed a large contribution of aromatic carbon, aliphatic carbon, carboxyl and carbonyl carbon, while the high temperature-derived biochars contained a large amount of aromatic carbon. Moreover, the wood-derived biochars produced at low heat treatment temperatures contained more lignin residues than grass-derived ones, probably due to the existence of high lignin content in the feedstock soures of wood-derived biochars. The results of the study would be useful for environmental application of biochars.

  2. First multimodal embolization particles visible on x-ray/computed tomography and magnetic resonance imaging.

    Science.gov (United States)

    Bartling, Soenke H; Budjan, Johannes; Aviv, Hagit; Haneder, Stefan; Kraenzlin, Bettina; Michaely, Henrik; Margel, Shlomo; Diehl, Steffen; Semmler, Wolfhard; Gretz, Norbert; Schönberg, Stefan O; Sadick, Maliha

    2011-03-01

    Embolization therapy is gaining importance in the treatment of malignant lesions, and even more in benign lesions. Current embolization materials are not visible in imaging modalities. However, it is assumed that directly visible embolization material may provide several advantages over current embolization agents, ranging from particle shunt and reflux prevention to improved therapy control and follow-up assessment. X-ray- as well as magnetic resonance imaging (MRI)-visible embolization materials have been demonstrated in experiments. In this study, we present an embolization material with the property of being visible in more than one imaging modality, namely MRI and x-ray/computed tomography (CT). Characterization and testing of the substance in animal models was performed. To reduce the chance of adverse reactions and to facilitate clinical approval, materials have been applied that are similar to those that are approved and being used on a routine basis in diagnostic imaging. Therefore, x-ray-visible Iodine was combined with MRI-visible Iron (Fe3O4) in a macroparticle (diameter, 40-200 μm). Its core, consisting of a copolymerized monomer MAOETIB (2-methacryloyloxyethyl [2,3,5-triiodobenzoate]), was coated with ultra-small paramagnetic iron oxide nanoparticles (150 nm). After in vitro testing, including signal to noise measurements in CT and MRI (n = 5), its ability to embolize tissue was tested in an established tumor embolization model in rabbits (n = 6). Digital subtraction angiography (DSA) (Integris, Philips), CT (Definition, Siemens Healthcare Section, Forchheim, Germany), and MRI (3 Tesla Magnetom Tim Trio MRI, Siemens Healthcare Section, Forchheim, Germany) were performed before, during, and after embolization. Imaging signal changes that could be attributed to embolization particles were assessed by visual inspection and rated on an ordinal scale by 3 radiologists, from 1 to 3. Histologic analysis of organs was performed. Particles provided a

  3. Magnetic resonance urography and X-ray urography findings of congenital megaureter.

    Science.gov (United States)

    Li, Tian-Ran; Du, Xiang-Ke; Huo, Tian-Long

    2011-06-01

    To observe the imaging findings of congenital megaureter in order to enhance the understanding of this disease. Image data of 5 patients with congenital megaureter and 2 misdiagnosed patients were analyzed, and image findings of congenital megaureter were summarized.Elscint Prestig 2.0T superconductive magnetic resonance urography (MRU) with conventional sequence (spin-echo, T1WI560 ms/16 ms; fast spin-echo, T2WI 9600 ms/96 ms ) was performed. Raw data were acquired with fastspin-echo sequence from heavy T2-weighted image (9600 ms/120 ms). Post-processing method of MRU was the maximum intensity projection with three-dimensional reconstruction in the workstation. Intravenous pyelography (IVP) was conducted, in which X-rayfilms were taken 7 minutes, 15 minutes, and 30 minutes after injecting contrast agent, exceptthat in 2 patients the films were taken delayed at 60 and 90 minutes .X-ray retrograde pyelography was performed on 2 patients, successful in one butfailed in the other. The dilated ureter showed hypointensity on T1-weighted images and hyperintensity on T2-weighted images in conventional MRI. The mass wall was intact, uniform in thickness, and showing hypointensity on T1-weighted and T2-weighted images. The MRU images showed a retroperitoneal mass appearing as an elongated tubular cystic structure spreading from kidney to bladder. MRU also revealed dilated calices and renal pelvis, pelviureteric obstruction, and renal duplication. The main signs of congenital megaureter in X-urography was significant dilatation of ureter, or normal renal pelvis with ureter dilatation, hydronephrosis, deformity, and displacement. MRU with X-urography could visualizethe characteristics of congenital megaureter, including the dilation of renal pelvis and ureter, calculi, urinary tract duplication, and stenosis location. The two techniques can complement each other in disease diagnosis and provide more detailed information for preoperative treatment.

  4. Pelvimetry using magnetic resonance imaging. Comparison with X-ray pelvimetry

    Energy Technology Data Exchange (ETDEWEB)

    Kinugasa, Masato; Suzuki, Hiromi; Miyazaki, Yoshihiko [Amagasaki Cooperative Hospital, Hyogo (Japan)

    2000-03-01

    To evaluate the diagnostic value of magnetic resonance pelvimetry (MRP) in pregnant women at term in comparison with X-ray pelvimetry (X-P). The basic experiment revealed the accuracy of MRP to be satisfactory. Then MRP was performed in thirty-two pregnant women at term (27 with breech presentation and 5 with cephalic presentation) and five non-pregnant patients. Twenty-seven of the pregnant women and all of the non-pregnant patients had X-P simultaneously. Measured MRP and X-P pelvic diameters were compared. Measured diameters of the pelvic inlet (auteroposterior and transverse) were nearly the same with MRP and X-P. But the outlet antero-posterior diameters measured by MRP were smaller than those measured by X-P in twenty-five of twenty-seven women, by an average of 1.0 cm (p<0.001). This gap may result from the difference in posture during examination by means of MRP (supine) and X-P (standing, for lateral image). MRP may represent the actual state of pelvic outlet of women during labor on delivery tables or beds. Vaginal delivery was planned for 22 women with breech presentation who were considered to have an adequate pelvis. Eighteen (82%) of them had successful vaginal delivery and the four other patients had a cesarean section (C/S) due to arrest of labor. Three of four women with cephalic presentation who were suspected by MRP to have a contracted pelvis underwent C/S due to cephalopelvic disproportion. MRP may be a promising alternative to conventional X-P, because it can provide accurate measurements without the hazard of ionizing radiation. (author)

  5. Examination of funnel chests by X-ray and nuclear magnetic resonance tomography: First results and experiences

    Energy Technology Data Exchange (ETDEWEB)

    Raithel, H.J.; Hartung, M.; Gruennewig, B.; Willital, G.

    1983-01-01

    Funnel chest (pectus excavatum) is a congenital malformation of the thorax. Operative correction must presently be regarded as the treatment of choise. In addition to cosmetical and psychological reasons, there are mainly functional aspects justifying a surgery. The indication for surgery results mostly from the objective clinical-diagnostical findings. This article describes the efficiency of both X-ray computerized tomography and also nuclear magnetic resonance tomography (NMR-CAT) which has only recently been introduced to clinical diagnostics.

  6. Resonant inelastic scattering in dilute magnetic semiconductors by x-ray fluorescence spectroscopy

    Energy Technology Data Exchange (ETDEWEB)

    Lawniczak-Jablonska, K. [Lawrence Berkeley National Lab., CA (United States)]|[Institute of Physics, Warsaw (Poland); Jia, J.J.; Underwood, J.H. [Lawrence Berkeley National Lab., CA (United States)] [and others

    1997-04-01

    As modern, technologically important materials have become more complex, element specific techniques have become invaluable in studying the electronic structure of individual components from the system. Soft x-ray fluorescence (SXF) and absorption (SXA) spectroscopies provide a unique means of measuring element and angular momentum density of electron states, respectively, for the valence and conducting bands in complex materials. X-ray absorption and the decay through x-ray emission are generally assumed to be two independent one-photon processes. Recent studies, however have demonstrated that SXF excited near the absorption threshold generate an array of spectral features that depend on nature of materials, particularly on the localization of excited states in s and d-band solids and that these two processes can no be longer treated as independent. Resonant SXF offers thus the new way to study the dynamics of the distribution of electronic valence states in the presence of a hole which is bound to the electron low lying in the conduction band. This process can simulate the interaction between hole-electron pair in wide gap semiconductors. Therefore such studies can help in understanding of transport and optics phenomena in the wide gap semiconductors. The authors report the result of Mn and S L-resonant emission in Zn{sub 1{minus}x}Mn{sub x}S (with x=0.2 and 0.3) and MnS as the energy of exciting radiation is tuned across the Mn and S L{sub 3,2} absorption edge, along with the resonant excited spectra from elemental Mn as a reference.

  7. X-rays and magnetism.

    Science.gov (United States)

    Fischer, Peter; Ohldag, Hendrik

    2015-09-01

    Magnetism is among the most active and attractive areas in modern solid state physics because of intriguing phenomena interesting to fundamental research and a manifold of technological applications. State-of-the-art synthesis of advanced magnetic materials, e.g. in hybrid structures paves the way to new functionalities. To characterize modern magnetic materials and the associated magnetic phenomena, polarized x-rays have emerged as unique probes due to their specific interaction with magnetic materials. A large variety of spectroscopic and microscopic techniques have been developed to quantify in an element, valence and site-sensitive way properties of ferro-, ferri-, and antiferromagnetic systems, such as spin and orbital moments, and to image nanoscale spin textures and their dynamics with sub-ns time and almost 10 nm spatial resolution. The enormous intensity of x-rays and their degree of coherence at next generation x-ray facilities will open the fsec time window to magnetic studies addressing fundamental time scales in magnetism with nanometer spatial resolution. This review will give an introduction into contemporary topics of nanoscale magnetic materials and provide an overview of analytical spectroscopy and microscopy tools based on x-ray dichroism effects. Selected examples of current research will demonstrate the potential and future directions of these techniques.

  8. Magnetic structure of Ho{sub 2}CoGa{sub 8} determined by X-ray resonant magnetic scattering

    Energy Technology Data Exchange (ETDEWEB)

    Adriano, C., E-mail: cadriano@ifi.unicamp.b [Instituto de Fisica ' Gleb Wataghin' , UNICAMP, C. P. 6165, 13083-970 Campinas, SP (Brazil); Giles, C.; Coelho, L.N.; Faria, G.A.; Pagliuso, P.G. [Instituto de Fisica ' Gleb Wataghin' , UNICAMP, C. P. 6165, 13083-970 Campinas, SP (Brazil)

    2009-10-15

    We report the low temperature magnetic structure of the Ho{sub 2}CoGa{sub 8} intermetallic compound studied by X-ray magnetic scattering technique at the Brazilian Synchrotron Light Laboratory. We found that below T{sub N}=5.1K, Ho{sub 2}CoGa{sub 8} has a commensurate antiferromagnetic structure with a propagation vector eta{sup -}>=(1/2 ,1/2 ,1/2 ) and preliminary analysis indicated that the Ho magnetic moment points along the c-axis. The magnetic structure of this compound was obtained by measuring the strong dipolar resonant peak at the L{sub 3} edge using polarization analysis. The magnetic structure and properties Ho{sub 2}CoGa{sub 8} are found to be consistent with the general trend already seen for the Nd-, Tb-, and the Ce-based compounds from the R{sub m}M{sub n}In{sub 3m+2n} family (R=rare earth; M=Co, Rh, or Ir; m=1,2; n=0,1).

  9. Nanocrystalline tin oxide: Possible origin of its weak ferromagnetism deduced from nuclear magnetic resonance and X-ray photoelectron spectroscopies

    Science.gov (United States)

    Zhang, Feng; Lian, Yadong; Gu, Min; Yu, Ji; Tang, Tong B.; Sun, Jian; Zhang, Weiyi

    2016-09-01

    Nanocrystalline tin oxide was fabricated, with molar ratio O/Sn determined as 1.40, 1.55, 1.79, 1.92 and 1.96 from X-ray photoelectron spectroscopy. They displayed weak ferromagnetism, the sample with O/Sn = 1.55 showing the maximum saturation magnetization reaching almost 8 ×10-3 emu /g at room temperature. 119Sn nuclear magnetic resonance allowed the deduction, based on four resolved resonance peaks, that their Sn ions had four possible coordination numbers, namely 3, 4, 5 and 6. The relative fraction of 4-coordinated cations was the one found to bear positive linear correlation with saturation magnetization of the sample. It is surmised that magnetism in tin oxide results mainly from 4-coordination Sn ions, of valance about +3, as estimated from the binding energies of their 3d photoelectron emission levels.

  10. Perpendicular Magnetic Anisotropy and Induced Magnetic Structures of Pt Layers in the Fe/Pt Multilayers Investigated by Resonant X-ray Magnetic Scattering

    Science.gov (United States)

    Lee, Mihee; Takechi, Ryota; Hosoito, Nobuyoshi

    2017-02-01

    Depth distribution of the magnetization induced in the paramagnetic Pt layers of Fe/Pt multilayers was investigated by resonant X-ray magnetic scattering (RXMS) near the Pt L3 absorption edge. Two samples with different perpendicular magnetic anisotropy (PMA) were chosen for RXMS measurements. The magnetic depth profile of the Pt layer was determined in the magnetic saturation state of the Fe magnetization with the sample of weak PMA. The magnetization process of the Pt layer was investigated with the sample of moderate PMA. It is found that the Pt atoms near the interface region have a perpendicular component of the induced magnetization even in the saturation state of the Fe magnetization, suggesting that the PMA of Fe/Pt multilayers originates from the Pt atoms near the interface region. Concerning the magnetization process, the induced Pt magnetization is not proportional to the Fe magnetization. This implies a complicated magnetizing mechanism of the Pt layer by the Fe magnetization.

  11. Ground state of the quasi-1D compound BaVS3 resolved by resonant magnetic x-ray scattering.

    Science.gov (United States)

    Leininger, Ph; Ilakovac, V; Joly, Y; Schierle, E; Weschke, E; Bunau, O; Berger, H; Pouget, J-P; Foury-Leylekian, P

    2011-04-22

    Resonant magnetic x-ray scattering near the vanadium L2,3-absorption edges has been used to investigate the low temperature magnetic structure of high quality BaVS3 single crystals. Below T(N)=31  K, the strong resonance revealed a triple-incommensurate magnetic ordering at the wave vector (0.226   0.226   ξ) in hexagonal notation, with ξ=0.033. The azimuthal-angle dependence of the scattering signal and time-dependent density functional theory simulations indicate an antiferromagnetic order within the ab plane with the spins polarized along a in the monoclinic structure.

  12. Employing soft x-ray resonant magnetic scattering to study domain sizes and anisotropy in Co/Pd multilayers

    Science.gov (United States)

    Bagschik, Kai; Frömter, Robert; Bach, Judith; Beyersdorff, Björn; Müller, Leonard; Schleitzer, Stefan; Berntsen, Magnus Hârdensson; Weier, Christian; Adam, Roman; Viefhaus, Jens; Schneider, Claus Michael; Grübel, Gerhard; Oepen, Hans Peter

    2016-10-01

    It is demonstrated that the magnetic diffraction pattern of the isotropic disordered maze pattern is well described utilizing a gamma distribution of domain sizes in a one-dimensional model. From the analysis, the mean domain size and the shape parameter of the distribution are obtained. The model reveals an average domain size that is significantly different from the value that is determined from the peak position of the structure factor in reciprocal space. As a proof of principle, a wedge-shaped (Cot Å/Pd10 Å)8 multilayer film, that covers the thickness range of the spin-reorientation transition, has been used. By means of soft x-ray resonant magnetic scattering (XRMS) and imaging techniques the thickness-driven evolution of the magnetic properties of the cobalt layers is explored. It is shown that minute changes of the domain pattern concerning domain size and geometry can be investigated and analyzed due to the high sensitivity and lateral resolution of the XRMS technique. The latter allows for the determination of the magnetic anisotropies of the cobalt layers within a thickness range of a few angstroms.

  13. Classification of materials using nuclear magnetic resonance dispersion and/or x-ray absorption

    Science.gov (United States)

    Espy, Michelle A.; Matlashov, Andrei N.; Schultz, Larry J.; Volegov, Petr L.; Urbaitis, Algis; Sandin, Henrik; Yoder, Jacob; Surko, Stephen

    2017-01-31

    Methods for determining the identity of a substance are provided. A classification parameter set is defined to allow identification of substances that previously could not be identified or to allow identification of substances with a higher degree of confidence. The classification parameter set may include at least one of relative nuclear susceptibility (RNS) or an x-ray linear attenuation coefficient (LAC). RNS represents the density of hydrogen nuclei present in a substance relative to the density of hydrogen nuclei present in water. The extended classification parameter set may include T.sub.1, T.sub.2, and/or T.sub.1.rho. as well as at least one additional classification parameter comprising one of RNS or LAC. Values obtained for additional classification parameters as well as values obtained for T.sub.1, T.sub.2, and T.sub.1.rho. can be compared to known classification parameter values to determine whether a particular substance is a known material.

  14. Classification of materials using nuclear magnetic resonance dispersion and/or x-ray absorption

    Energy Technology Data Exchange (ETDEWEB)

    Espy, Michelle A.; Matlashov, Andrei N.; Schultz, Larry J.; Volegov, Petr L.; Urbaitis, Algis; Sandin, Henrik; Yoder, Jacob; Surko, Stephen

    2017-01-31

    Methods for determining the identity of a substance are provided. A classification parameter set is defined to allow identification of substances that previously could not be identified or to allow identification of substances with a higher degree of confidence. The classification parameter set may include at least one of relative nuclear susceptibility (RNS) or an x-ray linear attenuation coefficient (LAC). RNS represents the density of hydrogen nuclei present in a substance relative to the density of hydrogen nuclei present in water. The extended classification parameter set may include T.sub.1, T.sub.2, and/or T.sub.1.rho. as well as at least one additional classification parameter comprising one of RNS or LAC. Values obtained for additional classification parameters as well as values obtained for T.sub.1, T.sub.2, and T.sub.1.rho. can be compared to known classification parameter values to determine whether a particular substance is a known material.

  15. Magnetic and electronic orderings in orthorhombic RMnO3 (R=Tm, Lu) studied by resonant soft x-ray powder diffraction

    Science.gov (United States)

    Garganourakis, M.; Bodenthin, Y.; de Souza, R. A.; Scagnoli, V.; Dönni, A.; Tachibana, M.; Kitazawa, H.; Takayama-Muromachi, E.; Staub, U.

    2012-08-01

    Resonant soft x-ray powder diffraction experiments on orthorhombic TmMnO3 and LuMnO3 are presented. Experiments were performed in the vicinity of the Tm M5 and the Mn L2,3 edges to study the Tm and Mn magnetic moments, respectively. These experiments show that for the heavy rare-earth perovskite with an E-type ordered ground state, the Tm magnetic moments order already in the nonferroelectric incommensurate magnetic phase. Additionally, deviations from the collinear E-type Mn magnetic structure at low temperatures are found for both compounds. These experiments show the power of resonant soft x-ray diffraction, extended to polycrystalline 4f materials.

  16. Advanced characterization of pores and fractures in coals by nuclear magnetic resonance and X-ray computed tomography

    Institute of Scientific and Technical Information of China (English)

    2010-01-01

    This paper demonstrates capabilities of low-field nuclear magnetic resonance (NMR) and microfocus X-ray computed tomography (μCT) in advanced, nondestructive, and quantitative characterization of pore types, producible porosity, pore structure, and spatial disposition of pore-fractures in coals. Results show that the NMR transverse relaxation time (T2) at 0.5–2.5, 20–50, and >100 ms correspond to pores of <0.1 μm, >0.1 μm, and fractures, respectively. A much higher T2 spectrum peak reflects a much better development of pores (or fractures) corresponding to the T2, and vice versa. Three basic components in coals, i.e., the pores (or fractures), coal matrix, and minerals have their distinctive range of CT numbers. Among these, the CT number of pores is commonly less than 600 HU. The producible porosity, which is a determination of permeability, can be calculated by T2 cutoff value (T2C) of coal NMR. The coal pore structure can be efficiently estimated by the newly proposed "T2C based model". Finally, μCT scan was proven capable of modeling and spatial visualization of pores and fractures.

  17. Evaluation of magnetic resonance imaging (MRI) in diagnosis of acoustic neuroma. Comparative study with plain X-ray and CTs

    Energy Technology Data Exchange (ETDEWEB)

    Nomura, Kimihisa; Sakai, Makoto; Shinkawa, Atsushi; Miyake, Hirosato; Matsukawa, Junichi

    1987-11-01

    In order to find an approach to earlier and more acurate diagnosis of acoustic neuroma, a comparative evaluation of MRI, plain X-ray (Stenvers' projection), high resolution CT with or without Metrizamide enhancement and air-CT has been made in five clinical cases of acoustic neuroma. A paramagnetic contrast agent, Gadolinium-diethylenetriamine pentaacetic acid (Gd-DTPA), was used to enhance images resolution in two cases of acoustic neuroma. In MRI, the high singnal mass in the posterior fossa was smaller than 10 x 10 mm in 2 cases, 17 x 20 mm in 2 cases and 35 x 40 mm in one case. MRI revealed enlargement of the neurovascular bundle around the VII and VIII cranial nerves compatible with a diagnosis of acoustic neuroma in all 5 cases, and masses within the cerebellopontine angle were also disclosed. In 2 cases the image of equivocal acoustic neuromas was well enhanced, and these lesions were visualized after intravenous administration of Gd-DTPA. In one of the cases the acoustic neuroma was satisfactorily differentiated from the surrounding cystic lesion with the aid of a contrast medium. Magnetic resonance which uses no ionizing radiation seems to be innocuous and offers several advantages over other imaging methods and CT, which may produce an adverse reaction when a contrast medium is used in CT-cisternography. Further advancement of MR technology will offer greater assistance in differential diagnosis of lesions such as acoustic tumors or other cerebellopontine angle tumors.

  18. Magnetic resonance imaging and dual energy X-ray absorptiometry of the lumbar spine in professional wrestlers and untrained men.

    Science.gov (United States)

    Hu, M; Sheng, J; Kang, Z; Zou, L; Guo, J; Sun, P

    2014-08-01

    The aim of this study was to examine the relation between bone marrow adipose tissue (BMAT) and bone mineral density (BMD) of lumbar spine in male professional wrestlers and healthy untrained men. A total of 14 wrestlers (22.9±3.4 years) and 11 controls (24.4±1.6 years) were studied cross-sectionally. Body composition and BMD were measured by dual-energy X-ray absorptiometry. Magnetic resonance imaging of the lumbar spine was examined in a sagittal T1-weighted (T1-w) spin-echo (SE) sequence. The averaged bone marrow signal intensity (SI) of L2-L4 was related to the signal of an adjacent nondegenerative disk. Mean SI of T1-w SE in wrestlers was lower than controls (P=0.001), indicating L2-L4 BMAT in wrestlers was lower compared to controls. L2-L4 BMD in wrestlers was higher than controls (PBMAT and BMD was confirmed in this relatively small subject sample with narrow age range, which implies that exercise training is an important determinant of this association.

  19. Analysis of ovariectomy and estrogen effects on body composition in rats by X-ray and magnetic resonance imaging techniques.

    Science.gov (United States)

    Sharp, J C; Copps, J C; Liu, Q; Ryner, L N; Sebastian, R A; Zeng, G Q; Smith, S; Niere, J O; Tomanek, B; Sato, M

    2000-01-01

    Resistance of bone to fracture--bone strength--has been shown to depend on both the amount of bone and its architectural spatial organization. In vivo magnetic resonance (MR) techniques have the capability of imaging bone tissue, including the trabecular microarchitecture and the marrow composition. We have applied in vivo and ex vivo MR methods to the tibia in an ovariectomized rat model of osteoporosis. Specifically, in vivo high-resolution three-dimensional MR imaging and localized MRS were facilitated by specialized coils and high field magnets, resulting in enhanced sensitivity of detection. As a result, in vivo and ex vivo differences in marrow composition were found between sham-ovariectomized, ovariectomized, and ovariectomized animals treated with 17-beta-estradiol. Estrogen effects were detected in vivo 7 days after surgery (3 days into treatment) as a decrease in the tibial fat signal level. The in vivo effects of ovariectomy were observed 56 days after surgery as an increase in MR image fat signal level and spectral fat/water ratio in the proximal tibia. Ex vivo measurements of tibial marrow water signal discriminated clearly between the sham and ovariectomized groups and showed increased individual variations in the treatment group. Imaging further showed that the highest fat content is observed in the epiphysis. Computed tomography confirmed ovariectomy-induced loss of bone in the proximal tibial metaphysis compared with the sham group. This loss of cancellous bone with ovariectomy is consistent with the MR observations of increases in both fat and water in the metaphysis. These data showed that MR techniques complement X-ray techniques in the bone, water, and fat compositional analysis of the appendicular skeleton in response to ovariectomy and pharmacological treatment.

  20. Resonant soft X-ray magnetic scattering study of magnetic structures in La{sub 1.5}Ca{sub 0.5}CoO{sub 4}

    Energy Technology Data Exchange (ETDEWEB)

    Okamoto, J., E-mail: jun.okamoto@kek.jp [Condensed Matter Research Center, IMSS, KEK, 1-1 Oho, Ibaraki 305-0801 (Japan); Horigane, K. [WPI-AIMR, Tohoku University, 2-1-1 Katahira, Aoba-ku, Sendai, Miyagi 980-8577 (Japan); Nakao, H.; Amemiya, K.; Kubota, M.; Murakami, Y. [Condensed Matter Research Center, IMSS, KEK, 1-1 Oho, Ibaraki 305-0801 (Japan); Yamada, K. [WPI-AIMR, Tohoku University, 2-1-1 Katahira, Aoba-ku, Sendai, Miyagi 980-8577 (Japan)

    2011-04-15

    Using Co L{sub 2,3} resonant soft X-ray scattering measurement, we reveal that the magnetic orderings with q = (1/2, 0, 1/2) and (1/2, 0, 1) originate from different magnetic domains. Temperature dependence of the magnetic ordering peaks clearly shows that there is a finite difference between the transition temperatures of these magnetic orderings.

  1. Imaging characteristics of intraocular foreign bodies: a comparative study of plain film X-ray, computed tomography, ultrasound, and magnetic resonance imaging.

    Science.gov (United States)

    Modjtahedi, Bobeck S; Rong, Andrew; Bobinski, Mathew; McGahan, John; Morse, Lawrence S

    2015-01-01

    To determine the imaging features of common intraocular foreign bodies (IOFBs) and the ability to differentiate types of IOFBs. Four-mm IOFBs were inserted via through pars plana approach into cadaveric lamb eyes. Six metallic (aluminum, brass, copper, silver, steel, and lead) and seven nonmetallic (plastic [CF6 spectacle plastic and polyvinyl chloride pipe], glass [bottle glass and windshield glass], wood [dry and wet poplar], and stone [slate]) IOFBs were imaged using plain film x-ray, computed tomography scan, ultrasound, and magnetic resonance imaging (T1, T2, and gradient echo sequences). Plain film x-ray had limited ability to differentiate most IOFBs. Computed tomography findings can be divided into low attenuation objects (wood), moderate attenuation (CF6 spectacle plastic), high attenuation without surrounding artifact (polyvinyl chloride, slate, bottle glass, windshield glass, and aluminum), high attenuation with shadow artifact and minimal edge streak artifact (steel, brass, copper), and high attenuation with significant shadow artifact and prominent streak artifact (silver and lead). Density (in Hounsfield units) aided in differentiating the types of IOFBs. Gradient echo sequences on magnetic resonance imaging also held utility. Ultrasound images had considerable overlap in appearances. Imaging techniques can significantly aid in determining the IOFBs type, with computed tomography serving as the best initial modality. X-ray holds limited utility while ultrasound and magnetic resonance imaging are best reserved as adjunctive tests.

  2. Two-dimensional resonant magnetic soft X-ray scattering set-up for extreme sample environment.

    Science.gov (United States)

    Stanescu, Stefan; Mocuta, Cristian; Merlet, Frederic; Barbier, Antoine

    2013-01-01

    The newly built MagSAXS (magnetic small-angle X-ray scattering) set-up dedicated to the direct two-dimensional measurement of magnetic scattering using polarized synchrotron radiation in extreme sample environments is presented. Pure optical transport of the image is used to record the magnetic scattering with a two-dimensional CCD visible-light camera. The set-up is able to probe magnetic correlation lengths from the micrometer down to the nanometer scale. A detailed layout is presented along with preliminary results obtained at several beamlines at Synchrotron SOLEIL. The presented examples underline the wide range of possible applications spanning from correlation lengths determination to Fourier transform holography.

  3. EuTiO3 magnetic structure studied by neutron powder diffraction and resonant x-ray scattering

    Science.gov (United States)

    Scagnoli, Valerio; Allieta, Mattia; Walker, Helen; Scavini, Marco; Katsufuji, Takuro; Sagarna, Leyre; Zaharko, Oksana; Mazzoli, Claudio

    2012-09-01

    We combine neutron powder diffraction and x-ray single-crystal magnetic diffraction at the Eu L2 edge to scrutinize the magnetic motif of the Eu ions in magnetoelectric EuTiO3. Our measurements are consistent with an antiferromagnetic G-type pattern with the Eu magnetic moments ordering along the a,b-plane diagonal. Recent reports of a novel transition at 2.75 K with a flop of magnetic moments upon poling the sample in an electric field cannot be confirmed for a nonpoled sample. Our neutron diffraction data do not show any significant change of the structure below the Néel temperature. Magnetoelastic coupling, if present, is therefore expected to be negligible.

  4. Temperature and field dependent magnetization in a sub-μm patterned Co/FeRh film studied by resonant x-ray scattering

    Science.gov (United States)

    Lounis, Lounès; Spezzani, Carlo; Delaunay, Renaud; Fortuna, Franck; Obstbaum, Martin; Günther, Stefan; Back, Christian H.; Popescu, Horia; Vidal, Franck; Sacchi, Maurizio

    2016-05-01

    We studied the temperature and field dependence of the magnetization in a Co/FeRh/MgO(0 0 1) film patterned into a matrix of sub-μm sized rectangles, using element selective resonant scattering of polarized soft x-rays. We show that it is possible to reverse partially the magnetization of the Co layer in a thermal cycle that crosses the FeRh antiferromagnetic to ferromagnetic transition. Our results support interest in patterned Co/FeRh films and their potential for achieving temperature induced magnetization switching.

  5. Investigation of the commensurate magnetic structure in the heavy-fermion compound CePt2In7 using magnetic resonant x-ray diffraction

    Science.gov (United States)

    Gauthier, Nicolas; Wermeille, Didier; Casati, Nicola; Sakai, Hironori; Baumbach, Ryan E.; Bauer, Eric D.; White, Jonathan S.

    2017-08-01

    We investigated the magnetic structure of the heavy-fermion compound CePt2In7 below TN=5.34 (2 ) K using magnetic resonant x-ray diffraction at ambient pressure. The magnetic order is characterized by a commensurate propagation vector k1 /2=(1/2 ,1/2 ,1/2 ) with spins lying in the basal plane. Our measurements did not reveal the presence of an incommensurate order propagating along the high-symmetry directions in reciprocal space but cannot exclude other incommensurate modulations or weak scattering intensities. The observed commensurate order can be described equivalently by either a single-k structure or by a multi-k structure. Furthermore we explain how a commensurate-only ordering may explain the broad distribution of internal fields observed in nuclear quadrupolar resonance experiments [Sakai et al., Phys. Rev. B 83, 140408 (2011), 10.1103/PhysRevB.83.140408] that was previously attributed to an incommensurate order. We also report powder x-ray diffraction showing that the crystallographic structure of CePt2In7 changes monotonically with pressure up to P =7.3 GPa at room temperature. The determined bulk modulus B0=81.1 (3 ) GPa is similar to those of the Ce-115 family. Broad diffraction peaks confirm the presence of pronounced strain in polycrystalline samples of CePt2In7 . We discuss how strain effects can lead to different electronic and magnetic properties between polycrystalline and single crystal samples.

  6. Hyperpolarized (3)He magnetic resonance imaging: comparison with four-dimensional x-ray computed tomography imaging in lung cancer.

    Science.gov (United States)

    Mathew, Lindsay; Wheatley, Andrew; Castillo, Richard; Castillo, Edward; Rodrigues, George; Guerrero, Thomas; Parraga, Grace

    2012-12-01

    Pulmonary functional imaging using four-dimensional x-ray computed tomographic (4DCT) imaging and hyperpolarized (3)He magnetic resonance imaging (MRI) provides regional lung function estimates in patients with lung cancer in whom pulmonary function measurements are typically dominated by tumor burden. The aim of this study was to evaluate the quantitative spatial relationship between 4DCT and hyperpolarized (3)He MRI ventilation maps. Eleven patients with lung cancer provided written informed consent to 4DCT imaging and MRI performed within 11 ± 14 days. Hyperpolarized (3)He MRI was acquired in breath-hold after inhalation from functional residual capacity of 1 L hyperpolarized (3)He, whereas 4DCT imaging was acquired over a single tidal breath of room air. For hyperpolarized (3)He MRI, the percentage ventilated volume was generated using semiautomated segmentation; for 4DCT imaging, pulmonary function maps were generated using the correspondence between identical tissue elements at inspiratory and expiratory phases to generate percentage ventilated volume. After accounting for differences in image acquisition lung volumes ((3)He MRI: 1.9 ± 0.5 L ipsilateral, 2.3 ± 0.7 L contralateral; 4DCT imaging: 1.2 ± 0.3 L ipsilateral, 1.3 ± 0.4 L contralateral), there was no significant difference in percentage ventilated volume between hyperpolarized (3)He MRI (72 ± 11% ipsilateral, 79 ± 12% contralateral) and 4DCT imaging (74 ± 3% ipsilateral, 75 ± 4% contralateral). Spatial correspondence between 4DCT and (3)He MRI ventilation was evaluated using the Dice similarity coefficient index (ipsilateral, 86 ± 12%; contralateral, 88 ± 12%). Despite rather large differences in image acquisition breathing maneuvers, good spatial and significant quantitative agreement was observed for ventilation maps on hyperpolarized (3)He MRI and 4DCT imaging, suggesting that pulmonary regions with good lung function are similar between modalities in this small group of patients with

  7. Soft X-ray techniques to study mesoscale magnetism

    Energy Technology Data Exchange (ETDEWEB)

    Kortright, Jeffrey B.

    2003-06-26

    Heterogeneity in magnetization (M) is ubiquitous in modern systems. Even in nominally homogeneous materials, domains or pinning centers typically mediate magnetization reversal. Fundamental lengths determining M structure include the domain wall width and the exchange stiffness length, typically in the 4-400 nm range. Chemical heterogeneity (phase separation, polycrystalline microstructure, lithographic or other patterning, etc.) with length scales from nanometers to microns is often introduced to influence magnetic properties. With 1-2 nm wavelengths {lambda}, soft x-rays in principle can resolve structure down to {lambda}/2, and are well suited to study these mesoscopic length scales [1, 2]. This article highlights recent advances in resonant soft x-ray methods to resolve lateral magnetic structure [3], and discusses some of their relative merits and limitations. Only techniques detecting x-ray photons (rather than photo-electrons) are considered [4], since they are compatible with strong applied fields to probe relatively deeply into samples. The magneto-optical (MO) effects discovered by Faraday and Kerr were observed in the x-ray range over a century later, first at ''hard'' wavelengths in diffraction experiments probing interatomic magnetic structure [5]. In the soft x-ray range, magnetic linear [6] and circular [7] dichroism spectroscopies first developed that average over lateral magnetic structure. These large resonant MO effects enable different approaches to study magnetic structure or heterogeneity that can be categorized as microscopy or scattering [1]. Direct images of magnetic structure result from photo-emission electron microscopes [4, 8] and zone-plate microscopes [9, 10]. Scattering techniques extended into the soft x-ray include familiar specular reflection that laterally averages over structure but can provide depth-resolved information, and diffuse scattering and diffraction that provide direct information about lateral

  8. Early experience with X-ray magnetic resonance fusion for low-flow vascular malformations in the pediatric interventional radiology suite

    Energy Technology Data Exchange (ETDEWEB)

    Hwang, Tiffany J. [The Children' s Hospital of Philadelphia, Department of Radiology, Philadelphia, PA (United States); Keck School of Medicine of the University of Southern California, Los Angeles, CA (United States); Girard, Erin [Siemens Corporation, Corporate Technology, Princeton, NJ (United States); Shellikeri, Sphoorti; Vossough, Arastoo; Ho-Fung, Victor; Cahill, Anne Marie [The Children' s Hospital of Philadelphia, Department of Radiology, Philadelphia, PA (United States); Setser, Randolph [Siemens Medical Solutions USA, Inc., Hoffman Estates, IL (United States)

    2016-03-15

    This technical innovation describes our experience using an X-ray magnetic resonance fusion (XMRF) software program to overlay 3-D MR images on real-time fluoroscopic images during sclerotherapy procedures for vascular malformations at a large pediatric institution. Five cases have been selected to illustrate the application and various clinical utilities of XMRF during sclerotherapy procedures as well as the technical limitations of this technique. The cases demonstrate how to use XMRF in the interventional suite to derive additional information to improve therapeutic confidence with regards to the extent of lesion filling and to guide clinical management in terms of intraprocedural interventional measures. (orig.)

  9. Novel motor design for rotating anode x-ray tubes operating in the fringe field of a magnetic resonance imaging system

    Energy Technology Data Exchange (ETDEWEB)

    Lillaney, Prasheel; Pelc, Norbert [Department of Radiology, Stanford University, Stanford, California 94305 and Department of Bioengineering, Stanford University, Stanford, California 94305 (United States); Shin Mihye [Department of Radiology, Stanford University, Stanford, California 94305 and Department of Mechanical Engineering, Stanford University, Stanford, California 94305 (United States); Hinshaw, Waldo; Fahrig, Rebecca [Department of Radiology, Stanford University, Stanford, California 94305 (United States); Bennett, N. Robert [Department of Radiology, Stanford University, Stanford, California 94305 and Qualcomm MEMS Technologies, San Jose, California 95134 (United States)

    2013-02-15

    Purpose: Using hybrid x-ray/MR (XMR) systems for image guidance during interventional procedures could enhance the diagnosis and treatment of neurologic, oncologic, cardiovascular, and other disorders. The authors propose a close proximity hybrid system design in which a C-arm fluoroscopy unit is placed immediately adjacent to the solenoid magnet of a MR system with a minimum distance of 1.2 m between the x-ray and MR imaging fields of view. Existing rotating anode x-ray tube designs fail within MR fringe field environments because the magnetic fields alter the electron trajectories in the x-ray tube and act as a brake on the induction motor, reducing the rotation speed of the anode. In this study the authors propose a novel motor design that avoids the anode rotation speed reduction. Methods: The proposed design replaces the permanent magnet stator found in brushed dc motors with the radial component of the MR fringe field. The x-ray tube is oriented such that the radial component of the MR fringe field is orthogonal to the cathode-anode axis. Using a feedback position sensor and the support bearings as electrical slip rings, the authors use electrical commutation to eliminate the need for mechanical brushes and commutators. A vacuum compatible prototype of the proposed motor design was assembled, and its performance was evaluated at various operating conditions. The prototype consisted of a 3.1 in. diameter anode rated at 300 kHU with a ceramic rotor that was 5.6 in. in length and had a 2.9 in. diameter. The material chosen for all ceramic components was MACOR, a machineable glass ceramic developed by Corning Inc. The approximate weight of the entire assembly was 1750 g. The maximum rotation speed, angular acceleration, and acceleration time of the motor design were investigated, as well as the dependence of these parameters on rotor angular offset, magnetic field strength, and field orientation. The resonance properties of the authors' assembly were also

  10. Perpendicular Magnetic Anisotropy in Ultrathin Co/Ni Multilayer Films Studies with Ferromagnetic Resonance and Magnetic X-Ray Microspectroscopy

    Science.gov (United States)

    2012-06-28

    Element specific hysteresis measurements for n¼6 obtained at the Fe L3 edge with an out-of-plane applied field, showing a hard axis magnetic response...of the perpendicular magnetic anisotropy in these systems, XMCD spectroscopy and element-specific hysteresis loops were measured at beam line U4B at...Fig. 2(b) and (c) were measured by tuning the photon energy to the L3 edges of Co, Ni, and Fe and sweeping the out-of-plane magnetic field from an

  11. The Efficacy of Magnetic Resonance Imaging and X-Ray in the Evaluation of Response to Radiosynovectomy in Patients with Hemophilic Arthropathy

    Directory of Open Access Journals (Sweden)

    Tamer Özülker

    2011-08-01

    Full Text Available Objective: We aimed to assess the role of Magnetic Resonance Imaging (MRI and X-Ray in the evaluation of response to radiosynovectomy (RS in patients with hemophilic arthropathy. Material and Methods: Eleven patients who suffered from hemophilic arthropathy with a mean age of 11.7 (range between 7-15 were included in this study. 148-185 MBq Yttrium 90 silicate (Y-90 was administered intraarticularly to ten knee joints and one patient was treated with intraarticular 74 MBq Rhenium 186 (Re-186 injection into his ankle. Before radiosynovectomy, plain anteroposterior and lateral X-rays of the target joints were obtained by standard technique. The follow-up MRI and X-ray studies of the patients were done 6 months after RS. Pettersson hemophilic arthropathy scales were utilized to stage the condition of the joints on plain X-ray and classification of the investigated joints on MRI were done according to Denver score. The clinical assessment of the efficacy of the RS was made with the comparison of the average bleedings before and after the intervention. Results: During the 6-month follow-up period after RS, an improvement in number of hemarthrosis 75% or greater compared with the prior six months occurred in six joints (54.5%. The Pettersson scores worsened in 1/11 (9%, remained unchanged in 9/11 (81.8%, and improved in 1/11 (9% joints. At the 6-month follow-up, the MRI score worsened in one (9% and was unchanged in 10/11 joints (90.9%. Conclusion: MRI is a more sensitive tool than plain radiography for evaluating and follow-up of joint disease in persons with hemophilia, but both methods don’t show correlation with the therapeutic response. (MIRT 2011;20:38-44

  12. Novel motor design for rotating anode x-ray tubes operating in the fringe field of a magnetic resonance imaging system.

    Science.gov (United States)

    Lillaney, Prasheel; Shin, Mihye; Hinshaw, Waldo; Bennett, N Robert; Pelc, Norbert; Fahrig, Rebecca

    2013-02-01

    Using hybrid x-ray∕MR (XMR) systems for image guidance during interventional procedures could enhance the diagnosis and treatment of neurologic, oncologic, cardiovascular, and other disorders. The authors propose a close proximity hybrid system design in which a C-arm fluoroscopy unit is placed immediately adjacent to the solenoid magnet of a MR system with a minimum distance of 1.2 m between the x-ray and MR imaging fields of view. Existing rotating anode x-ray tube designs fail within MR fringe field environments because the magnetic fields alter the electron trajectories in the x-ray tube and act as a brake on the induction motor, reducing the rotation speed of the anode. In this study the authors propose a novel motor design that avoids the anode rotation speed reduction. The proposed design replaces the permanent magnet stator found in brushed dc motors with the radial component of the MR fringe field. The x-ray tube is oriented such that the radial component of the MR fringe field is orthogonal to the cathode-anode axis. Using a feedback position sensor and the support bearings as electrical slip rings, the authors use electrical commutation to eliminate the need for mechanical brushes and commutators. A vacuum compatible prototype of the proposed motor design was assembled, and its performance was evaluated at various operating conditions. The prototype consisted of a 3.1 in. diameter anode rated at 300 kHU with a ceramic rotor that was 5.6 in. in length and had a 2.9 in. diameter. The material chosen for all ceramic components was MACOR, a machineable glass ceramic developed by Corning Inc. The approximate weight of the entire assembly was 1750 g. The maximum rotation speed, angular acceleration, and acceleration time of the motor design were investigated, as well as the dependence of these parameters on rotor angular offset, magnetic field strength, and field orientation. The resonance properties of the authors' assembly were also evaluated to determine

  13. Resonant x-ray scattering in correlated systems

    CERN Document Server

    Ishihara, Sumio

    2017-01-01

    The research and its outcomes presented here is devoted to the use of x-ray scattering to study correlated electron systems and magnetism. Different x-ray based methods are provided to analyze three dimensional electron systems and the structure of transition-metal oxides. Finally the observation of multipole orderings with x-ray diffraction is shown.

  14. Resonant X-ray scattering in correlated systems

    Energy Technology Data Exchange (ETDEWEB)

    Murakami, Youichi [High Energy Accelerator Research Organization, Tsukuba, Ibaraki (Japan). Inst. of Materials Structure Science; Ishihara, Sumio (ed.) [Tohoku Univ., Sendai, Miyagi (Japan). Dept. of Physics

    2017-03-01

    The research and its outcomes presented here is devoted to the use of X-ray scattering to study correlated electron systems and magnetism. Different X-ray based methods are provided to analyze three dimensional electron systems and the structure of transition-metal oxides. Finally the observation of multipole orderings with X-ray diffraction is shown.

  15. X-ray detection using magnetic calorimeters

    Energy Technology Data Exchange (ETDEWEB)

    Schoenefeld, J. E-mail: e62@urz.uni-heidelberg.de; Enss, C.; Fleischmann, A.; Sollner, J.; Horst, K.; Adams, J.S.; Kim, Y.H.; Seidel, G.M.; Bandler, S.R

    2000-04-07

    Using a magnetic calorimeter, we have obtained an energy resolution of 13 eV in the detection of 6 keV X-rays. The calorimeter consisted of a 50 {mu}m diameter, 25 {mu}m thick Au sensor doped with 300 ppm Er. A 100x100 {mu}m square, 8 {mu}m thick Au absorber was attached to the sensor. At the operating temperature of 33 mK and with a field of 3 mT, the calorimeter had a heat capacity of 1.3x10{sup -12} J/K. With a magnetic calorimeter optimized for X-ray detection an order of magnitude improvement in resolution should be possible.

  16. PEGylated NaHoF4 nanoparticles as contrast agents for both X-ray computed tomography and ultra-high field magnetic resonance imaging.

    Science.gov (United States)

    Ni, Dalong; Zhang, Jiawen; Bu, Wenbo; Zhang, Chen; Yao, Zhenwei; Xing, Huaiyong; Wang, Jing; Duan, Fei; Liu, Yanyan; Fan, Wenpei; Feng, Xiaoyuan; Shi, Jianlin

    2016-01-01

    It is well-known that multimodal imaging can integrate the advantages of different imaging modalities by overcoming their individual limitations. As ultra-high field magnetic resonance imaging (MRI) will be inevitably used in future MRI/X-ray computed tomography (CT) scanner, it is highly expected to develop high-performance nano-contrast agents for ultra-high field MR and CT dual-modality imaging, which has not been reported yet. Moreover, specific behavior of nano-contrast agents for ultra-high field MRI is a challenging work and still remains unknown. Herein, a novel type of NaHoF4 nanoparticles (NPs) with varied particle sizes were synthesized and explored as high-performance dual-modality contrast agents for ultra-high field MR and CT imaging. The specific X-ray absorption and MR relaxivity enhancements with varied nanoparticle diameters (3 nm, 7 nm, 13 nm and 29 nm) under different magnetic field (1.5/3.0/7.0 T) are investigated. Based on experimental results and theoretical analysis, the Curie and dipolar relaxation mechanisms of NaHoF4 NPs are firstly separated. Our results will greatly promote the future medical translational development of the NaHoF4 nano-contrast agents for ultra-high field MR/CT dual-modality imaging applications. Copyright © 2015 Elsevier Ltd. All rights reserved.

  17. Non-destructive Analysis of Oil-Contaminated Soil Core Samples by X-ray Computed Tomography and Low-Field Nuclear Magnetic Resonance Relaxometry: a Case Study

    Science.gov (United States)

    Mitsuhata, Yuji; Nishiwaki, Junko; Kawabe, Yoshishige; Utsuzawa, Shin; Jinguuji, Motoharu

    2010-01-01

    Non-destructive measurements of contaminated soil core samples are desirable prior to destructive measurements because they allow obtaining gross information from the core samples without touching harmful chemical species. Medical X-ray computed tomography (CT) and time-domain low-field nuclear magnetic resonance (NMR) relaxometry were applied to non-destructive measurements of sandy soil core samples from a real site contaminated with heavy oil. The medical CT visualized the spatial distribution of the bulk density averaged over the voxel of 0.31 × 0.31 × 2 mm3. The obtained CT images clearly showed an increase in the bulk density with increasing depth. Coupled analysis with in situ time-domain reflectometry logging suggests that this increase is derived from an increase in the water volume fraction of soils with depth (i.e., unsaturated to saturated transition). This was confirmed by supplementary analysis using high-resolution micro-focus X-ray CT at a resolution of ∼10 μm, which directly imaged the increase in pore water with depth. NMR transverse relaxation waveforms of protons were acquired non-destructively at 2.7 MHz by the Carr–Purcell–Meiboom–Gill (CPMG) pulse sequence. The nature of viscous petroleum molecules having short transverse relaxation times (T2) compared to water molecules enabled us to distinguish the water-saturated portion from the oil-contaminated portion in the core sample using an M0–T2 plot, where M0 is the initial amplitude of the CPMG signal. The present study demonstrates that non-destructive core measurements by medical X-ray CT and low-field NMR provide information on the groundwater saturation level and oil-contaminated intervals, which is useful for constructing an adequate plan for subsequent destructive laboratory measurements of cores. PMID:21258437

  18. Multifunctional BaYbF5: Gd/Er upconversion nanoparticles for in vivo tri-modal upconversion optical, X-ray computed tomography and magnetic resonance imaging.

    Science.gov (United States)

    Li, Xiaolong; Yi, Zhigao; Xue, Zhenluan; Zeng, Songjun; Liu, Hongrong

    2017-06-01

    Development of high-quality upconversion nanoparticles (UCNPs) with combination of the merits of multiple molecular imaging techniques, such as, upconversion luminescence (UCL) imaging, X-ray computed tomography (CT), and magnetic resonance (MR) imaging, could significantly improve the accuracy of biological diagnosis. In this work, multifunctional BaYbF5: Gd/Er (50:2mol%) UCNPs were synthesized via a solvothermal method using oleic acid (OA) as surface ligands (denoted as OA-UCNPs). The OA-UCNPs were further treated by diluted HCl to form ligand-free UCNPs (LF-UCNPs) for later bioimaging applications. The cytotoxicity assay in HeLa cells shows low cell toxicity of these LF-UCNPs. Owing to the efficient UCL of BaYbF5: Gd/Er, the LF-UCNPs were successfully used as luminescent bioprobe in UCL bioimaging. And, X-ray CT imaging reveals that BaYbF5: Gd/Er UCNPs can act as potential contrast agents for detection of the liver and spleen in the live mice owing to the high-Z elements (e.g., Ba, Yb, and Gd) in host matrix. Moreover, with the addition of Gd, the as-designed UCNPs exhibit additional positive contrast enhancement in T1-weighted MR imaging. These findings demonstrate that BaYbF5: Gd/Er UCNPs are potential candidates for tri-modal imaging. Copyright © 2017 Elsevier B.V. All rights reserved.

  19. Conformational characterization of synapse-associated protein 97 by nuclear magnetic resonance and small-angle X-ray scattering shows compact and elongated forms.

    Science.gov (United States)

    Tully, Mark D; Grossmann, J Günter; Phelan, Marie; Pandelaneni, Sravan; Leyland, Mark; Lian, Lu-Yun

    2012-01-31

    Synapse-associated protein 97 (SAP97) is a membrane-associated guanylate kinase protein that interacts with other proteins such as ion channels, subunits of glutamate receptors, and other cytoskeletal proteins and molecular scaffolds. The molecular diversity of SAP97 results from alternative splicing at the N-terminus, and in the U1 and U5 regions. There are two main N-terminal isoforms: the β-isoform has an L27 domain, whereas in the α-isoform, this is replaced by a palmitoylation motif. We have used multiangle light scattering, nuclear magnetic resonance, and small-angle X-ray scattering studies to characterize the conformation of a truncated form of the β-isoform, hence mimicking the α-isoform. This paper provides a comprehensive view of the small-angle X-ray scattering data, and the resulting data show that the scattering data are consistent with the presence of an ensemble of forms in dynamic equilibrium, with two prominent populations of compact and extended forms, with R(g) values of 38 ± 7 Å (52%) and 70 ± 10 Å (37%), respectively. The data show that without the L27 domain, the conformation of SAP97 is biased toward the compact form. We propose a hypothesis in which the overall conformation of SAP97 is determined by the nature of the N-terminus, which may, in turn, influence the specific role of a particular splice variant.

  20. Direct Characterization of Kerogen By X-Ray And Solid-State **13C Nuclear Magnetic Resonance Methods

    Energy Technology Data Exchange (ETDEWEB)

    Keleman, S.R.; Afeworki, M.; Gorbaty, M.L.; Sansone, M.; Kwiatek, P.J.; Walters, C.C.; Freund, H.; Siskin, M.; Bence, A.E.; Curry, D.J.; Solum, M.; Pugmire, R.J.; Vandenbroucke, M.; Leblond, M.; Behar, F.

    2007-07-09

    A combination of solid-state {sup 13}C NMR, X-ray photoelectron spectroscopy (XPS) and sulfur X-ray absorption near edge structure (S-XANES) techniques are used to characterize organic oxygen, nitrogen, and sulfur species and carbon chemical/structural features in kerogens. The kerogens studied represent a wide range of organic matter types and maturities. A van Krevelen plot based on elemental H/C data and XPS derived O/C data shows the well established pattern for type I, type II, and type III kerogens. The anticipated relationship between the Rock-Eval hydrogen index and H/C is independent of organic matter type. Carbon structural and lattice parameters are derived from solid-state 13C NMR analysis. As expected, the amount of aromatic carbon, measured by both {sup 13}C NMR and XPS, increases with decreasing H/C. The correlation between aromatic carbon and Rock-Eval Tmax, an indicator of maturity, is linear for types II and IIIC kerogens, but each organic matter type follows a different relationship. The average aliphatic carbon chain length (Cn') decreases with an increasing amount of aromatic carbon in a similar manner across all organic matter types. The fraction of aromatic carbons with attachments (FAA) decreases, while the average number of aromatic carbons per cluster (C) increases with an increasing amount of aromatic carbon. FAA values range from 0.2 to 0.4, and C values range from 12 to 20 indicating that kerogens possess on average 2- to 5-ring aromatic carbon units that are highly substituted. There is basic agreement between XPS and 13C NMR results for the amount and speciation of organic oxygen. XPS results show that the amount of carbon oxygen single bonded species increases and carbonyl-carboxyl species decrease with an increasing amount of aromatic carbon. Patterns for the relative abundances of nitrogen and sulfur species exist regardless of the large differences in the total amount of organic nitrogen and sulfur seen in the kerogens. XPS

  1. Direct Characterization of Kerogen by X-ray and Solid-State [superscript 13]C Nuclear Magnetic Resonance Methods

    Energy Technology Data Exchange (ETDEWEB)

    Kelemen, S. R.; Afeworki, M.; Gorbaty, M.L.; Sansone, M.; Kwiatek, P.J.; Walters, C.C.; Freund, H.; Siskin, M.; Bence, A.E.; Curry, D.J.; Solum, M.; Pugmire, R.J.; Vandenbroucke, M.; Leblond, M.; Behar, F. (ExxonMobil); (ExxonMobil); (IFP); (Utah)

    2008-06-12

    A combination of solid-state {sup 13}C NMR, X-ray photoelectron spectroscopy (XPS) and sulfur X-ray absorption near edge structure (S-XANES) techniques are used to characterize organic oxygen, nitrogen, and sulfur species and carbon chemical/structural features in kerogens. The kerogens studied represent a wide range of organic matter types and maturities. A van Krevelen plot based on elemental H/C data and XPS derived O/C data shows the well established pattern for type I, type II, and type III kerogens. The anticipated relationship between the Rock-Eval hydrogen index and H/C is independent of organic matter type. Carbon structural and lattice parameters are derived from solid-state {sup 13}C NMR analysis. As expected, the amount of aromatic carbon, measured by both {sup 13}C NMR and XPS, increases with decreasing H/C. The correlation between aromatic carbon and Rock-Eval T{sub max}, an indicator of maturity, is linear for types II and IIIC kerogens, but each organic matter type follows a different relationship. The average aliphatic carbon chain length (Cn) decreases with an increasing amount of aromatic carbon in a similar manner across all organic matter types. The fraction of aromatic carbons with attachments (FAA) decreases, while the average number of aromatic carbons per cluster (C) increases with an increasing amount of aromatic carbon. FAA values range from 0.2 to 0.4, and C values range from 12 to 20 indicating that kerogens possess on average 2- to 5-ring aromatic carbon units that are highly substituted. There is basic agreement between XPS and {sup 13}C NMR results for the amount and speciation of organic oxygen. XPS results show that the amount of carbon oxygen single bonded species increases and carbonyl-carboxyl species decrease with an increasing amount of aromatic carbon. Patterns for the relative abundances of nitrogen and sulfur species exist regardless of the large differences in the total amount of organic nitrogen and sulfur seen in the

  2. High energy resolution off-resonant X-ray spectroscopy

    Energy Technology Data Exchange (ETDEWEB)

    Wojciech, Blachucki [Univ. of Fribourg (Switzerland). Dept. of Physics

    2015-10-16

    This work treats of the high energy resolution off-resonant X-ray spectroscopy (HEROS) method of determining the density of unoccupied electronic states in the vicinity of the absorption edge. HEROS is an alternative to the existing X-ray absorption spectroscopy (XAS) methods and opens the way for new studies not achievable before.

  3. Golimumab therapy-induced indicators of X-ray inflammation progression and magnitude according to magnetic resonance imaging evidence in patients with rheumatoid arthritis, ankylosing spondylitis, or psoriatic arthritis

    Directory of Open Access Journals (Sweden)

    Aleksandr Viktorovich Smirnov

    2013-01-01

    Full Text Available The paper gives data on the progression of X-ray and magnetic resonance imaging changes in the hand and foot joints of patients with rheumatoid arthritis and psoriatic arthropathy and in the axial skeleton of those with ankylosing spondylitis when golimumab is used. Golimumab therapy is shown to retard the progression of structural changes in the peripheral joints and vertebral column. There is a significant correlation between magnetic resonance imaging evidence and blood C-reactive protein concentrations.

  4. Diagnosis of initial changes in patients suffering from rheumatoid arthritis. A comparison between low-field magnetic resonance imaging, 3-phase bone scintigraphy and conventional X-ray

    Energy Technology Data Exchange (ETDEWEB)

    Hoepfner, S.; Dresel, S.; Weiss, M.; Hahn, K. [Klinik und Poliklinik fuer Nuklearmedizin, Klinikum der Ludwig-Maximilians-Univ. Innenstadt, Muenchen (Germany); Treitl, M.; Krolak, C.; Becker-Gaab, C. [Inst. fuer Klinische Radiologie, Klinikum der Ludwig-Maximilians-Univ. Innenstadt, Muenchen (Germany); Schattenkirchner, M. [Rheumaeinheit der Medizinischen Poliklinik, Klinikum der Ludwig-Maximilians-Univ. Innenstadt, Muenchen (Germany)

    2002-06-01

    Besides conventional X-rays, in the diagnostic work up of initial changes in patients suffering from rheumatoid arthritis (RA), 3-phase bone scintigraphy (3P-Sz) is as well established as magnetic resonance imaging (MRI). The aim of this study was to compare the diagnostic value of the newly developed low field MRI with the proven methods X-rays and 3P-Sz. Methods: 65 patients (47f, 18m; 20-86 yrs) were studied on a one day protocol with 3P-Sz (550 MBq Tc-99m DPD), MRI and X-rays of the hands. Images were visually analysed by two blinded nuclear medicine physicians and radiologists and classified as a) RA-typical, b) inflammatory, non-RA-typical and c) non inflammatory changes. All methods were compared to 3P-Sz as golden standard. Results: In comparison to 3P-Sz, low field MRI presents with almost equal sensitivity and specificity in rheumatoid-typical and inflammatory changes. Conventional X-rays revealed in arthritis-typical changes as well as in inflammatory changes a significantly lower sensitivity and also a lower negative predictive value while specificity equals the one of MRI. Quantitative analysis of 3P-Sz using ROI-technique unveiled significantly higher values in patients with rheumatoid arthritis than in those with no inflammatory changes. Conclusion: MRI represents an equally sensitive method in the initial diagnosis of rheumatoid-typical and inflammatory changes in the region of the hands as compared to the 3P-Sz. Besides the basic diagnosis with conventional X-rays, 3P-Sz is still the recommended method of choice to evaluate the whole body when RA is suspected. Additionally, quantitative analysis of the 3P-Sz using the ROI technique in the region of the hands reveals statistically significant results and should therefore be taken into account in the assessment of inflammatory changes. (orig.) [German] Zur Diagnostik initialer Veraenderungen bei rheumatoider Arthritis (RA) werden neben der Projektionsradiographie (PR) im bilddiagnostischen

  5. X-ray resonant magnetic scattering investigations of hexagonal multiferroics RMnO3 (R = Dy, Ho, Er)

    Energy Technology Data Exchange (ETDEWEB)

    Nandi, Shibabrata [Iowa State Univ., Ames, IA (United States)

    2009-01-01

    Electricity and magnetism were unified into a common subject by James Clerk Maxwell in the nineteenth century yielding the electromagnetic theory. Four equations govern the dynamics of electric charges and magnetic fields, commonly known as Maxwell's equations. Maxwell's equations demonstrate that an accelerated charged particle can produce magnetic fields and a time varying magnetic field can induce a voltage - thereby linking the two phenomena. However, in solids, electric and magnetic ordering are most often considered separately and usually with good reason: the electric charges of electrons and ions are responsible for the charge effects, whereas the electron spin governs magnetic properties.

  6. Adjacent segment disease after anterior cervical decompression and fusion: analysis of risk factors on X-ray and magnetic resonance imaging

    Institute of Scientific and Technical Information of China (English)

    Zhao Yanbin; Sun Yu; Zhou Feifei; Wang Shaobo; Zhang Fengshan; Pan Shengfa

    2014-01-01

    Background Adjacent segment disease (ASD) is common after cervical fusion.The aim of this study was to evaluate the risk factors for ASD on X-ray and magnetic resonance imaging (MRI).Methods Patients included in this study had received revision surgeries after developing symptomatic ASD following anterior decompression and fusion.A control group that had not developed ASD was matched 1:1 by follow-up time and fusion segments.Plate-to-disc distances (PDDs),developmental cervical canal stenosis on X-ray,cervical disc degeneration grading,and cervical disc bulge impingements on preoperative MRI were measured and compared between the ASD group and the control group.Results Thirty-four patients with complete radiographic data were included in the ASD group.The causative segments of ASD included nine cases of C3-4,18 cases of C4-5,three cases of C5-6,and four cases of C6-7.The ASD occurred at the upper adjacent segments in 26 patients and at the lower adjacent segments in eight patients.PDD distributions were similar between the ASD group and the control group.Developmental cervical canal stenosis was a risk factor for ASD,with an odd ratio value of 2.88.Preoperative cervical disc degenerations on MRI were similar between the ASD group and the control group.In the upper-level ASD group,the disc bulge impingement was (19.7±9.7)%,which was significantly higher than that of the control group of (11.8±4.8)%.Conclusions ASD was more likely to develop above the index level of fusion.Developmental cervical canal stenosis and greater disc bulge impingement may be risk factors for the development of ASD.

  7. Synthesis, Characterization, In Vitro Phantom Imaging, and Cytotoxicity of A Novel Graphene-Based Multimodal Magnetic Resonance Imaging - X-Ray Computed Tomography Contrast Agent.

    Science.gov (United States)

    Lalwani, Gaurav; Sundararaj, Joe Livingston; Schaefer, Kenneth; Button, Terry; Sitharaman, Balaji

    2014-06-14

    Graphene nanoplatelets (GNPs), synthesized using potassium permanganate-based oxidation and exfoliation followed by reduction with hydroiodic acid (rGNP-HI), have intercalated manganese ions within the graphene sheets, and upon functionalization with iodine, show excellent potential as biomodal contrast agents for magnetic resonance imaging (MRI) and computed tomography (CT). Structural characterization of rGNP-HI nanoparticles with low- and high-resolution transmission electron microscope (TEM) showed disc-shaped nanoparticles (average diameter, 200 nm, average thickness, 3 nm). Energy dispersive X-ray spectroscopy (EDX) analysis confirmed the presence of intercalated manganese. Raman spectroscopy and X-ray diffraction (XRD) analysis of rGNP-HI confirmed the reduction of oxidized GNPs (O-GNPs), absence of molecular and physically adsorbed iodine, and the functionalization of graphene with iodine as polyiodide complexes (I3(-) and I5(-)). Manganese and iodine content were quantified as 5.1 ± 0.5 and 10.54 ± 0.87 wt% by inductively-coupled plasma optical emission spectroscopy and ion-selective electrode measurements, respectively. In vitro cytotoxicity analysis, using absorbance (LDH assay) and fluorescence (calcein AM) based assays, performed on NIH3T3 mouse fibroblasts and A498 human kidney epithelial cells, showed CD50 values of rGNP-HI between 179-301 µg/ml, depending on the cell line and the cytotoxicity assay. CT and MRI phantom imaging of rGNP-HI showed high CT (approximately 3200% greater than HI at equimolar iodine concentration) and MRI (approximately 59% greater than equimolar Mn(2+) solution) contrast. These results open avenues for further in vivo safety and efficacy studies towards the development of carbon nanostructure-based multimodal MRI-CT contrast agents.

  8. Application of cervical arthroplasty with Bryan cervical disc:long-term X-ray and magnetic resonance imaging follow-up results

    Institute of Scientific and Technical Information of China (English)

    ZHAO Yan-bin; SUN Yu; CHEN Zhong-qiang; LIU Zhong-jun

    2010-01-01

    Background Cervical disc arthroplasty is a new technique for treating degenerative cervical disease. Its goal is to avoid the degeneration of adjacent levels by preserving motion at the treated level. The aims of this study were to evaluate the radiologic outcomes of Bryan cervical disc replacement and the degenerative status of adjacent segments.Methods Twenty-two patients at a single center underwent discectomy and implantation of Bryan cervical disc. The mean follow-up period was 60 months (57-69 months). Twenty patients underwent single-level arthroplasty and two underwent arthroplasty at two levels. The levels of surgery included C3/4 (3 levels), C4/5 (2 levels), C5/6 (18 levels) and C6/7 (1 level). Radiographic evaluation included dynamic X-ray examination and magnetic resonance imaging (MRI) at baseline and at final follow-up.Results On X-ray examination, the range of motion (ROM) at the operated level was 7.2° (2.5°-13.0°) at baseline and 7.8° (1.0°-15.0°) at final follow-up (P >0.05). Heterotopic ossification around the prosthesis was observed in eight levels,and two levels showed loss of motion (ROM <2°). MRI showed worsening by a grade at the upper level in 2/22 patients,and worsening by a grade at the lower level in 3/22, according to Miyazaki's classification. No further impingement of the ligamentum flavum into the spinal canal was observed at adjacent levels, though the disc bulge was slightly increased at both the adjacent upper and lower levels at final follow-up.Conclusions Arthroplasty using Bryan cervical disc prosthesis resulted in favorable radiologic outcomes in this study.Disc degeneration at adjacent levels may be postponed by this technique.

  9. Deconvoluting Protein (Unfolding Structural Ensembles Using X-Ray Scattering, Nuclear Magnetic Resonance Spectroscopy and Molecular Dynamics Simulation.

    Directory of Open Access Journals (Sweden)

    Alexandr Nasedkin

    Full Text Available The folding and unfolding of protein domains is an apparently cooperative process, but transient intermediates have been detected in some cases. Such (unfolding intermediates are challenging to investigate structurally as they are typically not long-lived and their role in the (unfolding reaction has often been questioned. One of the most well studied (unfolding pathways is that of Drosophila melanogaster Engrailed homeodomain (EnHD: this 61-residue protein forms a three helix bundle in the native state and folds via a helical intermediate. Here we used molecular dynamics simulations to derive sample conformations of EnHD in the native, intermediate, and unfolded states and selected the relevant structural clusters by comparing to small/wide angle X-ray scattering data at four different temperatures. The results are corroborated using residual dipolar couplings determined by NMR spectroscopy. Our results agree well with the previously proposed (unfolding pathway. However, they also suggest that the fully unfolded state is present at a low fraction throughout the investigated temperature interval, and that the (unfolding intermediate is highly populated at the thermal midpoint in line with the view that this intermediate can be regarded to be the denatured state under physiological conditions. Further, the combination of ensemble structural techniques with MD allows for determination of structures and populations of multiple interconverting structures in solution.

  10. Resonant and non-resonant X-ray scattering from GdB{sub 6}

    Energy Technology Data Exchange (ETDEWEB)

    Kuwahara, K. [Department of Physics, Faculty of Science, Tokyo Metropolitan University, Hachioji, Tokyo 192-0397 (Japan)]. E-mail: kuwahara@phys.metro-u.ac.jp; Yamamoto, R. [Department of Physics, Faculty of Science, Tokyo Metropolitan University, Hachioji, Tokyo 192-0397 (Japan); Kohgi, M. [Department of Physics, Faculty of Science, Tokyo Metropolitan University, Hachioji, Tokyo 192-0397 (Japan); Nakao, H. [Faculty of Science, Tohoku University, Sendai 980-8577 (Japan); Ishii, K. [Synchrotron Radiation Research Center, JAERI, Hyogo 679-5148 (Japan); Iwasa, K. [Faculty of Science, Tohoku University, Sendai 980-8577 (Japan); Murakami, Y. [Faculty of Science, Tohoku University, Sendai 980-8577 (Japan); Kunii, S. [Faculty of Science, Tohoku University, Sendai 980-8577 (Japan); Sagayama, H. [Photon Factory, Institute for Materials Structure Science, KEK, Tsukuba 305-0801 (Japan); Wakabayashi, Y. [Photon Factory, Institute for Materials Structure Science, KEK, Tsukuba 305-0801 (Japan); Sawa, H. [Photon Factory, Institute for Materials Structure Science, KEK, Tsukuba 305-0801 (Japan)

    2005-04-30

    We have performed resonant and non-resonant X-ray scattering on GdB{sub 6} to investigate the two successive phase transitions at T{sub N}={approx}15K and T*={approx}10K. Below T{sub N}, new superlattice reflection at the wave vector [141412], which is the same wave vector determined by the epithermal neutron diffraction, has been observed by X-ray scattering. In the temperature region between T* and T{sub N}, it was confirmed by the polarization analyses that the superlattice reflection is due to magnetic X-ray scattering. On the other hand, interestingly, the superlattice reflection below T* is mainly due to Thomson scattering. Unlike behavior expected from usual magnetoelastic effects, the wave vector of the lattice distortion is identical to that of the magnetic structure below T*.

  11. Trifunctional Polymeric Nanocomposites Incorporated with Fe₃O₄/Iodine-Containing Rare Earth Complex for Computed X-ray Tomography, Magnetic Resonance, and Optical Imaging.

    Science.gov (United States)

    Wang, Xin; Tu, Mengqi; Yan, Kai; Li, Penghui; Pang, Long; Gong, Ying; Li, Qing; Liu, Ruiqing; Xu, Zushun; Xu, Haibo; Chu, Paul K

    2015-11-11

    In this study, a novel polymerizable CT contrast agent integrating iodine with europium(III) has been developed by a facile and universal coordination chemistry method. The Fe3O4 nanoparticles are then incorporated into this iodine-containing europium complex by seed-emulsifier-free polymerization. The nanocomposites combining the difunctional complex and superparamagnetic Fe3O4 nanoparticles, which have uniform size dispersion and high encapsulation rate, are suitable for computed X-ray tomography (CT), magnetic resonance imaging (MRI), and optical imaging. They possess good paramagnetic properties with a maximum saturation magnetization of 2.16 emu/g and a transverse relaxivity rate of 260 mM(-1) s(-1), and they exhibit obvious contrast effects with an iodine payload less than 4.8 mg I/mL. In the in vivo optical imaging assessment, vivid fluorescent dots can be observed in the liver and spleen by two-photon confocal scanning laser microscopy (CLSM). All the results showed that nanocomposites as polymeric trifunctional contrast agents have great clinical potential in CT, MR, and optical imaging.

  12. Electron cyclotron resonance ion source plasma characterization by X-ray spectroscopy and X-ray imaging

    Energy Technology Data Exchange (ETDEWEB)

    Mascali, David, E-mail: davidmascali@lns.infn.it; Castro, Giuseppe; Celona, Luigi; Neri, Lorenzo; Gammino, Santo [INFN–Laboratori Nazionali del Sud, Via S. Sofia 62, 95125 Catania (Italy); Biri, Sándor; Rácz, Richárd; Pálinkás, József [Institute for Nuclear Research (Atomki), Hungarian Academy of Sciences, Bem tér 18/c, H-4026 Debrecen (Hungary); Caliri, Claudia [INFN–Laboratori Nazionali del Sud, Via S. Sofia 62, 95125 Catania (Italy); Università degli Studi di Catania, Dip.to di Fisica e Astronomia, via Santa Sofia 64, 95123 Catania (Italy); Romano, Francesco Paolo [INFN–Laboratori Nazionali del Sud, Via S. Sofia 62, 95125 Catania (Italy); CNR, Istituto per i Beni Archeologici e Monumentali, Via Biblioteca 4, 95124 Catania (Italy); Torrisi, Giuseppe [INFN–Laboratori Nazionali del Sud, Via S. Sofia 62, 95125 Catania (Italy); Università Mediterranea di Reggio Calabria, DIIES, Via Graziella, I-89100 Reggio Calabria (Italy)

    2016-02-15

    An experimental campaign aiming to investigate electron cyclotron resonance (ECR) plasma X-ray emission has been recently carried out at the ECRISs—Electron Cyclotron Resonance Ion Sources laboratory of Atomki based on a collaboration between the Debrecen and Catania ECR teams. In a first series, the X-ray spectroscopy was performed through silicon drift detectors and high purity germanium detectors, characterizing the volumetric plasma emission. The on-purpose developed collimation system was suitable for direct plasma density evaluation, performed “on-line” during beam extraction and charge state distribution characterization. A campaign for correlating the plasma density and temperature with the output charge states and the beam intensity for different pumping wave frequencies, different magnetic field profiles, and single-gas/gas-mixing configurations was carried out. The results reveal a surprisingly very good agreement between warm-electron density fluctuations, output beam currents, and the calculated electromagnetic modal density of the plasma chamber. A charge-coupled device camera coupled to a small pin-hole allowing X-ray imaging was installed and numerous X-ray photos were taken in order to study the peculiarities of the ECRIS plasma structure.

  13. Comparative characterization of the data of magnetic resonance imaging, X-ray and clinical studies of the hand and foot joints in patients with early psoriatic arthritis

    Directory of Open Access Journals (Sweden)

    Svetlana Olegovna Krasnenko

    2013-01-01

    Full Text Available The clinical manifestations of psoriatic arthritis (PsA at its early stage may be inadequately informative. In this connection, radiological techniques, such as magnetic resonance imaging (MRI and X-ray study of peripheral joints, in addition to clinical examination are of paramount importance in the diagnosis of early PsA. Objective: To compare the data of clinical examination and various imaging methods (MRI and X-ray of the hand and foot joints in early peripheral PsA. Subjects and methods. The trial included 45 patients (14 men and 31 women; mean age 42.08±13.7 years; median PsA duration 1 year [range 0.55 to 2] with early peripheral PsA without previous therapy with disease-modifying antirheumatic drugs (DMARDs, who met the CASPAR criteria (2006. A standard clinical examination was performed and the activity of peripheral arthritis and the presence of enthesitis and dactylitis were determined in the patients. Not later than 2 days after the clinical examination, a standard X-ray examination of the hands and feet in the direct projection and MRI of the same areas were made. Results. When included into the study, the entire group of patients was found to have a moderate PsA by DAS; its median was 3.12 [2.21 to 3.89]. Cutaneous PsA was noted in 40 patients; 5 persons had a family history of PsA; one female patient had ungual PsA only. In the study group, the clinical signs of enthesitis in the tendon attachments at different sites were revealed in 33 (75.3% patients. Dactylitis was found in 34 (75% patients. The clinical examination showed inflammatory changes in the hand and foot joints in 36 (80% and 38 (84% patients, respectively; while MRT revealed them in 31 (69% and 32 (71% patients. Hand MRI displayed arthritis of the proximal interpha-langeal (PIP, metacarpophalangeal (MCP, and distal interphalangeal (DIP joints in 27 (87%, 21 (68%, and 12 (40% of the 31 patients, respectively. Foot MRI exhibited MCP, PIP, and DIP joint arthritis in

  14. First Principles Calculations for X-ray Resonant Spectra and Elastic Properties

    Energy Technology Data Exchange (ETDEWEB)

    Lee, Yongbin [Iowa State Univ., Ames, IA (United States)

    2004-01-01

    In this thesis, we discuss applications of first principles methods to x-ray resonant spectra and elastic properties calculation. We start with brief reviews about theoretical background of first principles methods, such as density functional theory, local density approximation (LDA), LDA+U, and the linear augmented plane wave (LAPW) method to solve Kohn-Sham equations. After that we discuss x-ray resonant scattering (XRMS), x-ray magnetic circular dichroism (XMCD) and the branching problem in the heavy rare earths Ledges. In the last chapter we discuss the elastic properties of the second hardest material AlMgB14.

  15. The Influence of Magnetic Resonance Imaging Findings of Degenerative Disease on Dual-Energy X-ray Absorptiometry Measurements in Middle-Aged Men

    Energy Technology Data Exchange (ETDEWEB)

    Donescu, O.S.; Battie, M.C.; Videman, T. [Faculty of Rehabilitation Medicine and Dept. of Physical Therapy, Univ. of Alberta (Canada)

    2007-02-15

    Purpose: To examine degenerative features based on magnetic resonance imaging (MRI) measurements at the lumbar spine in relation to dual-energy X-ray absorptiometry (DXA), and to investigate whether bone mineral density (BMD) is reflected in the substitution of bone trabecular structure by fat at the vertebral body level indicated by MRI T1 relaxation time, endplate concavity, and hypertrophic (osteophytes and endplate sclerosis) MRI findings. Material and Methods: The sample for this cross-sectional study was composed of 102 subjects, 35-70 years old, from a population-based cohort. Data collection included DXA in the anterior-posterior projection at the L1-L4 vertebrae and right femoral neck, and MRI of the lumbar spine in the midsagittal plane. Results: Age, vertebral signal intensity, osteophytes, and endplate concavity collectively explained 20% of the variance in spine BMD. Conclusion: The study findings suggest that degenerative findings based on MRI measurements at the lumbar spine have an influence on bone assessment using DXA. Therefore, an overall bone assessment such as DXA might not offer an accurate measure of BMD.

  16. Characterization of very young mineral phases of bone by solid state 31phosphorus magic angle sample spinning nuclear magnetic resonance and X-ray diffraction.

    Science.gov (United States)

    Roberts, J E; Bonar, L C; Griffin, R G; Glimcher, M J

    1992-01-01

    The properties of bone mineral change with age and maturation. Several investigators have suggested the presence of an initial or "precursor" calcium phosphate phase to help explain these differences. We have used solid state 31P magic angle sample spinning (MASS) nuclear magnetic resonance (NMR) and X-ray radial distribution function (RDF) analyses to characterize 11- and 17-day-old embryonic chick bone and fractions obtained from them by density fractionation. Density fractionation provides samples of bone containing Ca-P solid-phase deposits even younger and more homogeneous with respect to the age of mineral than the calcium phosphate (Ca-P) deposits in the whole bone samples. The analytical techniques yield no evidence for any distinct phase other than the poorly crystalline hydroxyapatite phase characteristic of mature bone mineral. In particular, there is no detectable crystalline brushite [DCPD, CaHPO4 2H2O less than 1%] or amorphous calcium phosphate (less than 8-10%) in the most recently formed bone mineral. A sizeable portion of the phosphate groups exist as HPO4(2-) in a brushite (DCPD)-like configuration. These acid phosphate moieties are apparently incorporated into the apatitic lattice. The most likely site for the brushite-like configuration is probably on the surface of the crystals.

  17. X-ray fluorescence microscopy demonstrates preferential accumulation of a vanadium-based magnetic resonance imaging contrast agent in murine colonic tumors.

    Science.gov (United States)

    Mustafi, Devkumar; Ward, Jesse; Dougherty, Urszula; Bissonnette, Marc; Hart, John; Vogt, Stefan; Karczmar, Gregory S

    2015-01-01

    Contrast agents that specifically enhance cancers on magnetic resonance imaging (MRI) will allow earlier detection. Vanadium-based chelates (VCs) selectively enhance rodent cancers on MRI, suggesting selective uptake of VCs by cancers. Here we report x-ray fluorescence microscopy (XFM) of VC uptake by murine colon cancer. Colonic tumors in mice treated with azoxymethane/dextran sulfate sodium were identified by MRI. Then a gadolinium-based contrast agent and a VC were injected intravenously; mice were sacrificed and colons sectioned. VC distribution was sampled at 120 minutes after injection to evaluate the long-term accumulation. Gadolinium distribution was sampled at 10 minutes after injection due to its rapid washout. XFM was performed on 72 regions of normal and cancerous colon from five normal mice and four cancer-bearing mice. XFM showed that all gadolinium was extracellular, with similar concentrations in colon cancers and normal colon. In contrast, the average VC concentration was twofold higher in cancers versus normal tissue (p < .002). Cancers also contained numerous "hot spots" with intracellular VC concentrations sixfold higher than the concentration in normal colon (p < .0001). No hot spots were detected in normal colon. This is the first direct demonstration that VCs selectively accumulate in cancer cells and thus may improve cancer detection.

  18. PEGylated hybrid ytterbia nanoparticles as high-performance diagnostic probes for in vivo magnetic resonance and X-ray computed tomography imaging with low systemic toxicity.

    Science.gov (United States)

    Liu, Zhen; Pu, Fang; Liu, Jianhua; Jiang, Liyan; Yuan, Qinghai; Li, Zhengqiang; Ren, Jinsong; Qu, Xiaogang

    2013-05-21

    Novel nanoparticulate contrast agents with low systemic toxicity and inexpensive character have exhibited more advantages over routinely used small molecular contrast agents for the diagnosis and prognosis of disease. Herein, we designed and synthesized PEGylated hybrid ytterbia nanoparticles as high-performance nanoprobes for X-ray computed tomography (CT) imaging and magnetic resonance (MR) imaging both in vitro and in vivo. These well-defined nanoparticles were facile to prepare and cost-effective, meeting the criteria as a biomedical material. Compared with routinely used Iobitridol in clinic, our PEG-Yb2O3:Gd nanoparticles could provide much significantly enhanced contrast upon various clinical voltages ranging from 80 kVp to 140 kVp owing to the high atomic number and well-positioned K-edge energy of ytterbium. By the doping of gadolinium, our nanoparticulate contrast agent could perform perfect MR imaging simultaneously, revealing similar organ enrichment and bio-distribution with the CT imaging results. The super improvement in imaging efficiency was mainly attributed to the high content of Yb and Gd in a single nanoparticle, thus making these nanoparticles suitable for dual-modal diagnostic imaging with a low single-injection dose. In addition, detailed toxicological study in vitro and in vivo indicated that uniformly sized PEG-Yb2O3:Gd nanoparticles possessed excellent biocompatibility and revealed overall safety.

  19. Correlation of X-ray computed tomography with quantitative nuclear magnetic resonance methods for pre-clinical measurement of adipose and lean tissues in living mice.

    Science.gov (United States)

    Metzinger, Matthew N; Miramontes, Bernadette; Zhou, Peng; Liu, Yueying; Chapman, Sarah; Sun, Lucy; Sasser, Todd A; Duffield, Giles E; Stack, M Sharon; Leevy, W Matthew

    2014-10-08

    Numerous obesity studies have coupled murine models with non-invasive methods to quantify body composition in longitudinal experiments, including X-ray computed tomography (CT) or quantitative nuclear magnetic resonance (QMR). Both microCT and QMR have been separately validated with invasive techniques of adipose tissue quantification, like post-mortem fat extraction and measurement. Here we report a head-to-head study of both protocols using oil phantoms and mouse populations to determine the parameters that best align CT data with that from QMR. First, an in vitro analysis of oil/water mixtures was used to calibrate and assess the overall accuracy of microCT vs. QMR data. Next, experiments were conducted with two cohorts of living mice (either homogenous or heterogeneous by sex, age and genetic backgrounds) to assess the microCT imaging technique for adipose tissue segmentation and quantification relative to QMR. Adipose mass values were obtained from microCT data with three different resolutions, after which the data were analyzed with different filter and segmentation settings. Strong linearity was noted between the adipose mass values obtained with microCT and QMR, with optimal parameters and scan conditions reported herein. Lean tissue (muscle, internal organs) was also segmented and quantified using the microCT method relative to the analogous QMR values. Overall, the rigorous calibration and validation of the microCT method for murine body composition, relative to QMR, ensures its validity for segmentation, quantification and visualization of both adipose and lean tissues.

  20. Resonant soft X-ray fluorescence spectra of molecules

    Energy Technology Data Exchange (ETDEWEB)

    Nordgren, J.; Glans, P.; Gunnelin, K.; Guo, J.; Skytt, P.; Saathe, C.; Wassdahl, N. [Uppsala Univ. (Sweden). Dept. of Phys.

    1997-08-01

    A review is presented of some recent advancements in resonant soft X-ray fluorescence spectroscopy applied to molecules. The concept of inelastic scattering is discussed for molecules with an element of symmetry, which introduces degeneracy or near-degeneracy of core excited states. The potential of the symmetry selection rules associated with resonant X-ray fluorescence is illustrated in studies of electronic structure as well as molecular dynamics. The use of polarized photons for exciting X-ray emission is discussed, and examples are presented where anisotropy of X-ray emission provides more detailed information. A brief section discusses the experimental considerations relevant for the spectroscopic technique. (orig.) With 013 figs., 28 refs.

  1. Magnetic X-Ray Scattering with Synchrotron Radiation

    DEFF Research Database (Denmark)

    Moncton, D. E.; Gibbs, D.; Bohr, Jakob

    1986-01-01

    With the availability of high-brilliance synchrotron radiation from multiple wigglers, magnetic X-ray scattering has become a powerful new probe of magnetic structure and phase transitions. Similar to the well-established magnetic neutron scattering technique, magnetic X-ray scattering methods have...... many complementary advantages. A brief review is presented of the history of magnetic X-ray scattering as well as recent results obtained in studies of the rare-earth magnet holmium with emphasis on instrumentational aspects. In particular, the development of a simple polarization analyzer...

  2. Band structure approach to the resonant x-ray scattering

    OpenAIRE

    Elfimov, I. S.; Skorikov, N. A.; Anisimov, V. I.; Sawatzky, G.A.

    2001-01-01

    We study the resonance behaviour of the forbidden 600 and 222 x-ray Bragg peaks in Ge using LDA band structure methods. These Bragg peaks remain forbidden in the resonant dipole scattering approximation even taking into account the non local nature of the band states. However they become allowed at resonance if the eigenstates of the unoccupied conduction band involve a hybridization of p like and d like atomic states. We show that the energy dependence of the resonant behaviour, including th...

  3. Femtosecond X-ray magnetic circular dichroism absorption spectroscopy at an X-ray free electron laser

    Energy Technology Data Exchange (ETDEWEB)

    Higley, Daniel J., E-mail: dhigley@stanford.edu; Yuan, Edwin [SLAC National Accelerator Laboratory, 2575 Sand Hill Road, Menlo Park, California 94025 (United States); Department of Applied Physics, Stanford University, Stanford, California 94305 (United States); Hirsch, Konstantin; Dakovski, Georgi L.; Jal, Emmanuelle; Lutman, Alberto A.; Coslovich, Giacomo; Hart, Philip; Hoffmann, Matthias C.; Mitra, Ankush; Moeller, Stefan; Ohldag, Hendrik; Seaberg, Matthew; Stöhr, Joachim; Nuhn, Heinz-Dieter; Reid, Alex H.; Dürr, Hermann A.; Schlotter, William F. [SLAC National Accelerator Laboratory, 2575 Sand Hill Road, Menlo Park, California 94025 (United States); Liu, Tianmin; MacArthur, James P. [SLAC National Accelerator Laboratory, 2575 Sand Hill Road, Menlo Park, California 94025 (United States); Department of Physics, Stanford University, Stanford, California 94305 (United States); and others

    2016-03-15

    X-ray magnetic circular dichroism spectroscopy using an X-ray free electron laser is demonstrated with spectra over the Fe L{sub 3,2}-edges. The high brightness of the X-ray free electron laser combined with high accuracy detection of incident and transmitted X-rays enables ultrafast X-ray magnetic circular dichroism studies of unprecedented sensitivity. This new capability is applied to a study of all-optical magnetic switching dynamics of Fe and Gd magnetic sublattices in a GdFeCo thin film above its magnetization compensation temperature.

  4. Enhanced x-rays from resonant betatron oscillations in laser wakefield with external wigglers

    Science.gov (United States)

    Zhang, Z. M.; Zhang, B.; Hong, W.; Yu, M. Y.; Deng, Z. G.; Teng, J.; He, S. K.; Gu, Y. Q.

    2016-11-01

    Generation of ultra-short betatron x-rays by laser-accelerated electron beams is of great research interest as it has many applications. In this paper, we propose a scheme for obtaining bright betatron x-rays by applying external wiggler magnetic field in the laser wakefield to resonantly drive the betatron oscillations of the accelerated electrons therein. This results in a significant enhancement of the betatron oscillation amplitude and generation of bright x-rays with high photon energy. The scheme is demonstrated using two-dimensional particle-in-cell simulation and discussed using a simple analytical model.

  5. The prediction of total skeletal muscle mass in a Caucasian population - comparison of Magnetic resonance imaging (MRI) and Dual-energy X-ray absorptiometry (DXA).

    Science.gov (United States)

    Geisler, Corinna; Pourhassan, Maryam; Braun, Wiebke; Schweitzer, Lisa; Müller, Manfred J

    2017-03-01

    Dual-energy X-ray (DXA) is an alternative to magnetic resonance imaging (MRI) to measure skeletal muscle mass. DXA assesses lean body mass (LBM), and MRI measures skeletal muscle mass (SMM). Kim et al. (Am J Clin Nutr 2002; 76: 378; J Appl Physiol (1985) 2004; 97: 655) developed MRI-based algorithms to estimate whole-body SMM by DXA. These algorithms were based on an ethnically mixed study population (Kim et al., Am J Clin Nutr 2002; 76: 378; J Appl Physiol (1985) 2004; 97: 655). It is unclear whether Kim's algorithms are accurate in an exclusive Caucasian population. The aim of our study was to validate Kim's equation in a Caucasian population of 346 subjects. SMMMRI was assessed using MRI, and LBM and BMCDXA were measured by DXA and fat mass (FMADP ) by air-displacement plethysmographie (ADP). SMMMRI and predicted SMM were highly correlated (r = 0·944; P<0·05). The standard error of estimate of the regression equation was 2·4 kg. However, Bland-Altman plots showed a significant (P<0·001) systematic bias between SMMMRI (median 25·1 kg; IQ 20·2-31·1 kg) and predicted SMM (median 26·3 kg; IQ 22·6-33·0 kg), overestimating SMM by 9·8%. Multiple regression analyses showed that weight explained 4·4% of the variance in the differences between SMMMRI and predicted SMM with the major part unexplained. Kim's algorithm has a systematic unexplained bias and is not recommended in Caucasians.

  6. Correlation of X-Ray Computed Tomography with Quantitative Nuclear Magnetic Resonance Methods for Pre-Clinical Measurement of Adipose and Lean Tissues in Living Mice

    Directory of Open Access Journals (Sweden)

    Matthew N. Metzinger

    2014-10-01

    Full Text Available Numerous obesity studies have coupled murine models with non-invasive methods to quantify body composition in longitudinal experiments, including X-ray computed tomography (CT or quantitative nuclear magnetic resonance (QMR. Both microCT and QMR have been separately validated with invasive techniques of adipose tissue quantification, like post-mortem fat extraction and measurement. Here we report a head-to-head study of both protocols using oil phantoms and mouse populations to determine the parameters that best align CT data with that from QMR. First, an in vitro analysis of oil/water mixtures was used to calibrate and assess the overall accuracy of microCT vs. QMR data. Next, experiments were conducted with two cohorts of living mice (either homogenous or heterogeneous by sex, age and genetic backgrounds to assess the microCT imaging technique for adipose tissue segmentation and quantification relative to QMR. Adipose mass values were obtained from microCT data with three different resolutions, after which the data were analyzed with different filter and segmentation settings. Strong linearity was noted between the adipose mass values obtained with microCT and QMR, with optimal parameters and scan conditions reported herein. Lean tissue (muscle, internal organs was also segmented and quantified using the microCT method relative to the analogous QMR values. Overall, the rigorous calibration and validation of the microCT method for murine body composition, relative to QMR, ensures its validity for segmentation, quantification and visualization of both adipose and lean tissues.

  7. Screening in resonant X-ray emission of molecules

    DEFF Research Database (Denmark)

    Ågren, Hans; Luo, Yi; Gelmukhanov, Faris

    1996-01-01

    We explore the effects of screening in resonant X-ray emission from molecules by means of unconstrained multi-configurational self-consistent field optimizations of each state involved in the resonant and nonresonant X-ray processes. It is found that, although screening can produce shifts...... in transition energies of a few eV, its effect on the transition intensities is relatively minor. Using results from the investigated molecules, we find that the screening is quite dependent on the type of molecule - saturated versus unsaturated - and on the core site, but depends little on the particular core...

  8. International workshop on resonant X-ray scattering in electrically-ordered systems

    Energy Technology Data Exchange (ETDEWEB)

    Collins, S.P.; Pettifer, R.F.; Laundy, D.; Ishida, K.; Kokubun, J.; Giles, C.; Yokaichiya, F.; Song, C.; Lee, K.B.; Ji, S.; Koo, J.; Park, Y.J.; Kim, J.Y.; Park, J.H.; Shin, H.J.; Rhyee, J.S.; Oh, B.H.; Cho, B.K.; Wilkins Stuart, B.; Paixao, J.A.; Caciuffo, R.; Javorsky, P.; Wastin, F.; Rebizant, J.; Detlefs, C.; Bernheoft, N.; Lander, G.H.; Bombardi, A.; Bergevin, F. de; Matteo, S. di; Paolasini, L.; Rodriguez-Carvajal, J.; Carretta, P.; Millet, P.; Caciuffo, R.; Goff, J.P.; Deen, P.P.; Lee, S.; Stunault, A.; Brown, S.; Mannix, D.; McIntyre, G.J.; Ward, R.C.C.; Wells, M.R.; Lorenzo, J.E.; Joly, Y.; Nazarenko, E.; Staub, U.; Srajer, G.; Haskel, D.; Choi, Y.; Lee, D.R.; Lang, J.C.; Meersschaut, J.; Jiang, J.S.; Bader, S.D.; Bouchenoire, L.; Brown, S.D.; Beesley, A.; Herring, A.; Thomas, M.; Thompson, P.; Langridge, S.; Stirling, W.G.; Mirone, A.; Lander, G.; Wilkins, S.; Ward, R.C.C.; Wells, M.R.; Zochowski, S.W.; Garcia, J.; Subias, G.; Blasco, J.; Sanchez, M.C.; Proietti, M.G.; Lovesey, S.W.; Dmitrienko, V.E.; Ovchinnikova, E.N.; Ishida, K.; Kokubun, J.; Kirfel, A.; Collins, S.P.; Laundy, D.; Oreshko, A.P.; Strange, P.; Horne, M.; Arola, E.; Winter, H.; Szotek, Z.; Temmerman, W.M.; Igarashi, J.; Usuda, M.; Takahashi, M.; Matteo, S. di; Bernhoeft, N.; Hill, J.P.; Lang, J.C.; McWhan, D.; Lee, D.R.; Haskel, D.; Srajer, G.; Hatton Peter, D.; Katsumata, K.; Braithwaite, D

    2004-07-01

    The research field of Resonant X-ray Scattering (RXS) has achieved tremendous progress in the last years. Nowadays RXS is rapidly becoming the crucial technique for investigating the subtleties of microscopic magnetism in systems where the ground state properties reflect a delicate balance between several different correlated processes. The aim of this workshop is to discuss present and future possibilities for RXS investigations of electronic order, including studies of charge, magnetic, and multipolar ordered states. The sessions will cover experimental and theoretical aspects of hard and soft X-ray resonant scattering from single crystals and thin films. This document gathers the summaries of the presentations.

  9. Simultaneous surface plasmon resonance and x-ray absorption spectroscopy

    Science.gov (United States)

    Serrano, A.; Rodríguez de la Fuente, O.; Collado, V.; Rubio-Zuazo, J.; Monton, C.; Castro, G. R.; García, M. A.

    2012-08-01

    We present an experimental setup for the simultaneous measurement of surface plasmon resonance (SPR) and x-ray absorption spectroscopy (XAS) on metallic thin films at a synchrotron beamline. The system allows measuring in situ and in real time the effect of x-ray irradiation on the SPR curves to explore the interaction of x-rays with matter. It is also possible to record XAS spectra while exciting SPR in order to study changes in the films induced by the excitation of surface plasmons. Combined experiments recording simultaneously SPR and XAS curves while scanning different parameters can be also carried out. The relative variations in the SPR and XAS spectra that can be detected with this setup range from 10-3 to 10-5, depending on the particular experiment.

  10. Simultaneous Surface Plasmon Resonance and X-ray Absorption Spectroscopy

    CERN Document Server

    Serrano, A; Collado, V; Rubio-Zuazo, J; Monton, C; Castro, G; García, M A

    2012-01-01

    We present here an experimental set-up to perform simultaneously measurements of surface plasmon resonance (SPR) and X-ray absorption spectroscopy (XAS) in a synchrotron beamline. The system allows measuring in situ and in real time the effect of X-ray irradiation on the SPR curves to explore the interaction of X-rays with matter. It is also possible to record XAS spectra while exciting SPR in order to detect the changes in the electronic configuration of thin films induced by the excitation of surface plasmons. Combined experiments recording simultaneously SPR and XAS curves while scanning different parameters can be carried out. The relative variations in the SPR and XAS spectra that can be detected with this set-up ranges from 10-3 to 10-5, depending on the particular experiment.

  11. Simultaneous surface plasmon resonance and x-ray absorption spectroscopy

    Energy Technology Data Exchange (ETDEWEB)

    Serrano, A. [Instituto de Ceramica y Vidrio (ICV-CSIC), Cantoblanco, 28049 Madrid (Spain); Departamento de Fisica de Materiales, Universidad Complutense de Madrid, 28040 Madrid (Spain); Rodriguez de la Fuente, O. [Departamento de Fisica de Materiales, Universidad Complutense de Madrid, 28040 Madrid (Spain); Collado, V.; Rubio-Zuazo, J.; Castro, G. R. [SpLine, Spanish CRG Beamline at the ESRF, F-38043 Grenoble, Cedex 09, France and Instituto de Ciencia de Materiales de Madrid, (ICMM-CSIC), Cantoblanco, 28049 Madrid (Spain); Monton, C. [Department of Physics and Center for Advanced Nanoscience, University of California San Diego, La Jolla, California 92093 (United States); Garcia, M. A. [Instituto de Ceramica y Vidrio (ICV-CSIC), Cantoblanco, 28049 Madrid (Spain); IMDEA Nanociencia, Cantoblanco, 28049 Madrid (Spain)

    2012-08-15

    We present an experimental setup for the simultaneous measurement of surface plasmon resonance (SPR) and x-ray absorption spectroscopy (XAS) on metallic thin films at a synchrotron beamline. The system allows measuring in situ and in real time the effect of x-ray irradiation on the SPR curves to explore the interaction of x-rays with matter. It is also possible to record XAS spectra while exciting SPR in order to study changes in the films induced by the excitation of surface plasmons. Combined experiments recording simultaneously SPR and XAS curves while scanning different parameters can be also carried out. The relative variations in the SPR and XAS spectra that can be detected with this setup range from 10{sup -3} to 10{sup -5}, depending on the particular experiment.

  12. Bright circularly polarized soft X-ray high harmonics for X-ray magnetic circular dichroism

    Science.gov (United States)

    Fan, Tingting; Grychtol, Patrik; Knut, Ronny; Hernández-García, Carlos; Hickstein, Daniel D.; Zusin, Dmitriy; Gentry, Christian; Dollar, Franklin J.; Mancuso, Christopher A.; Hogle, Craig W.; Kfir, Ofer; Legut, Dominik; Carva, Karel; Ellis, Jennifer L.; Dorney, Kevin M.; Chen, Cong; Shpyrko, Oleg G.; Fullerton, Eric E.; Cohen, Oren; Oppeneer, Peter M.; Milošević, Dejan B.; Becker, Andreas; Jaroń-Becker, Agnieszka A.; Popmintchev, Tenio; Murnane, Margaret M.; Kapteyn, Henry C.

    2015-01-01

    We demonstrate, to our knowledge, the first bright circularly polarized high-harmonic beams in the soft X-ray region of the electromagnetic spectrum, and use them to implement X-ray magnetic circular dichroism measurements in a tabletop-scale setup. Using counterrotating circularly polarized laser fields at 1.3 and 0.79 µm, we generate circularly polarized harmonics with photon energies exceeding 160 eV. The harmonic spectra emerge as a sequence of closely spaced pairs of left and right circularly polarized peaks, with energies determined by conservation of energy and spin angular momentum. We explain the single-atom and macroscopic physics by identifying the dominant electron quantum trajectories and optimal phase-matching conditions. The first advanced phase-matched propagation simulations for circularly polarized harmonics reveal the influence of the finite phase-matching temporal window on the spectrum, as well as the unique polarization-shaped attosecond pulse train. Finally, we use, to our knowledge, the first tabletop X-ray magnetic circular dichroism measurements at the N4,5 absorption edges of Gd to validate the high degree of circularity, brightness, and stability of this light source. These results demonstrate the feasibility of manipulating the polarization, spectrum, and temporal shape of high harmonics in the soft X-ray region by manipulating the driving laser waveform. PMID:26534992

  13. Bright circularly polarized soft X-ray high harmonics for X-ray magnetic circular dichroism.

    Science.gov (United States)

    Fan, Tingting; Grychtol, Patrik; Knut, Ronny; Hernández-García, Carlos; Hickstein, Daniel D; Zusin, Dmitriy; Gentry, Christian; Dollar, Franklin J; Mancuso, Christopher A; Hogle, Craig W; Kfir, Ofer; Legut, Dominik; Carva, Karel; Ellis, Jennifer L; Dorney, Kevin M; Chen, Cong; Shpyrko, Oleg G; Fullerton, Eric E; Cohen, Oren; Oppeneer, Peter M; Milošević, Dejan B; Becker, Andreas; Jaroń-Becker, Agnieszka A; Popmintchev, Tenio; Murnane, Margaret M; Kapteyn, Henry C

    2015-11-17

    We demonstrate, to our knowledge, the first bright circularly polarized high-harmonic beams in the soft X-ray region of the electromagnetic spectrum, and use them to implement X-ray magnetic circular dichroism measurements in a tabletop-scale setup. Using counterrotating circularly polarized laser fields at 1.3 and 0.79 µm, we generate circularly polarized harmonics with photon energies exceeding 160 eV. The harmonic spectra emerge as a sequence of closely spaced pairs of left and right circularly polarized peaks, with energies determined by conservation of energy and spin angular momentum. We explain the single-atom and macroscopic physics by identifying the dominant electron quantum trajectories and optimal phase-matching conditions. The first advanced phase-matched propagation simulations for circularly polarized harmonics reveal the influence of the finite phase-matching temporal window on the spectrum, as well as the unique polarization-shaped attosecond pulse train. Finally, we use, to our knowledge, the first tabletop X-ray magnetic circular dichroism measurements at the N4,5 absorption edges of Gd to validate the high degree of circularity, brightness, and stability of this light source. These results demonstrate the feasibility of manipulating the polarization, spectrum, and temporal shape of high harmonics in the soft X-ray region by manipulating the driving laser waveform.

  14. Magnetically Confined Wind Shocks in X-rays - a Review

    CERN Document Server

    ud-Doula, Asif

    2015-01-01

    A subset (~ 10%) of massive stars present strong, globally ordered (mostly dipolar) magnetic fields. The trapping and channeling of their stellar winds in closed magnetic loops leads to magnetically confined wind shocks (MCWS), with pre-shock flow speeds that are some fraction of the wind terminal speed. These shocks generate hot plasma, a source of X-rays. In the last decade, several developments took place, notably the determination of the hot plasma properties for a large sample of objects using XMM-Newton and Chandra, as well as fully self-consistent MHD modelling and the identification of shock retreat effects in weak winds. Despite a few exceptions, the combination of magnetic confinement, shock retreat and rotation effects seems to be able to account for X-ray emission in massive OB stars. Here we review these new observational and theoretical aspects of this X-ray emission and envisage some perspectives for the next generation of X-ray observatories.

  15. Frontiers in imaging magnetism with polarized x-rays

    Directory of Open Access Journals (Sweden)

    Peter eFischer

    2015-01-01

    Full Text Available Although magnetic imaging with polarized x-rays is a rather young scientific discipline, the various types of established x-ray microscopes have already taken an important role in state-of-the-art characterization of the properties and behavior of spin textures in advanced materials. The opportunities ahead will be to obtain in a unique way indispensable multidimensional information of the structure, dynamics and composition of scientifically interesting and technologically relevant magnetic materials.

  16. The effect of water on the structure and dynamics of spider silk and silk-like polymers studied by magnetic resonance and x-ray diffraction

    Science.gov (United States)

    Yang, Zhitong

    Due to its unique combination of tensile strength and elasticity, the dragline silk of the orb-weaving spider Nephila clavipes has attracted much attention. Most importantly, it has a high energy to break that is unparalleled in other fibers. Though the basis for the strength of the silk fiber has been uncovered, the molecular reason of the fiber's large shrinkage in water is unknown. This has been a major hurdle in the practical applications of the fiber, and to any man-made copy of this material. Small-angle X-ray scattering (SAXS) is used to probe of the long-range structures in the semicrystalline silk. Scattering patterns of wet and dry samples indicate that the crystalline regions stack along the fiber axis to form lamellar structures. These structures are sparsely dispersed in a softer matrix with a long spacing of 8.4 nm. This spacing increases reversibly by 4% when fibers are stretched by 10%, and shrinks to 5.8 nm when fibers shrink 45% in length on wetting. Solid-state nuclear magnetic resonance (NMR) experiments are performed to reveal the microscopic details of the dynamics in the silk. Cross-polarization magic-angle spinning 13C NMR demonstrates that a substantial fraction of the glycine, glutamine, tyrosine, serine, and leucine residues experience dramatic increases in the rate of large-amplitude reorientation at the protein backbone when fibers are wet. Variable temperature deuterium NMR measurements were carried out on silk samples that incorporate leucine deuterated at the methyl group. Results show that only a subset of these leucine residues is strongly affected by water. Quantitative analysis and chemical considerations suggest that the highly conserved YGGLGS(N)QGAGR blocks, only found in the dragline silk protein, play a major role in the supercontraction process. Protein sequences are proposed to produce artificial spider silk with similar mechanical properties, but without the undesired phenomenon of supercontraction. The spinning and

  17. Multidimensional resonant nonlinear spectroscopy with coherent broadband x-ray pulses

    Science.gov (United States)

    Bennett, Kochise; Zhang, Yu; Kowalewski, Markus; Hua, Weijie; Mukamel, Shaul

    2016-12-01

    New x-ray free electron laser (XFEL) and high harmonic generation (HHG) light sources are capable of generating short and intense pulses that make x-ray nonlinear spectroscopy possible. Multidimensional spectroscopic techniques, which have long been used in the nuclear magnetic resonance, infrared, and optical regimes to probe the electronic structure and nuclear dynamics of molecules by sequences of short pulses with variable delays, can thus be extended to the attosecond x-ray regime. This opens up the possibility of probing core-electronic structure and couplings, the real-time tracking of impulsively created valence-electronic wavepackets and electronic coherences, and monitoring ultrafast processes such as nonadiabatic electron-nuclear dynamics near conical-intersection crossings. We survey various possible types of multidimensional x-ray spectroscopy techniques and demonstrate the novel information they can provide about molecules.

  18. Longitudinal detection of ferromagnetic resonance using x-ray transmission measurements

    Energy Technology Data Exchange (ETDEWEB)

    Boero, G.; Rusponi, S. [Ecole Polytechninque Federale de Lausanne (EPFL), CH-1015 Lausanne (Switzerland); Kavich, J.; Rizzini, A. Lodi [Centre d' Investigacio en Nanociencia i Nanotecnologia (ICN-CSIC), E-08193 Bellaterra, Barcelona (Spain); Piamonteze, C.; Nolting, F. [Swiss Light Source (SLS), Paul Scherrer Institut, CH-5232 Villigen (Switzerland); Tieg, C. [European Synchrotron Radiation Facility (ESRF), F-38043 Grenoble (France); Thiele, J.-U. [Seagate Technology, 47010 Kato Road, Fremont, California 94538 (United States); Gambardella, P. [Centre d' Investigacio en Nanociencia i Nanotecnologia (ICN-CSIC), E-08193 Bellaterra, Barcelona (Spain); Institucio Catalana de Recerca i Estudis Avancats (ICREA), E-08100 Barcelona (Spain)

    2009-12-15

    We describe a setup for the x-ray detection of ferromagnetic resonance in the longitudinal geometry using element-specific transmission measurements. Thin magnetic film samples are placed in a static magnetic field collinear with the propagation direction of a polarized soft x-ray beam and driven to ferromagnetic resonance by a continuous wave microwave magnetic field perpendicular to it. The transmitted photon flux is measured both as a function of the x-ray photon energy and as a function of the applied static magnetic field. We report experiments performed on a 15 nm film of doped Permalloy (Ni{sub 73}Fe{sub 18}Gd{sub 7}Co{sub 2}) at the L{sub 3}/L{sub 2}-edges of Fe, Co, and Ni. The achieved ferromagnetic resonance sensitivity is about 0.1 monolayers/{radical}(Hz). The obtained results are interpreted in the framework of a conductivity tensor based formalism. The factors limiting the sensitivity as well as different approaches for the x-ray detection of ferromagnetic resonance are discussed.

  19. Longitudinal detection of ferromagnetic resonance using x-ray transmission measurements.

    Science.gov (United States)

    Boero, G; Rusponi, S; Kavich, J; Rizzini, A Lodi; Piamonteze, C; Nolting, F; Tieg, C; Thiele, J-U; Gambardella, P

    2009-12-01

    We describe a setup for the x-ray detection of ferromagnetic resonance in the longitudinal geometry using element-specific transmission measurements. Thin magnetic film samples are placed in a static magnetic field collinear with the propagation direction of a polarized soft x-ray beam and driven to ferromagnetic resonance by a continuous wave microwave magnetic field perpendicular to it. The transmitted photon flux is measured both as a function of the x-ray photon energy and as a function of the applied static magnetic field. We report experiments performed on a 15 nm film of doped Permalloy (Ni(73)Fe(18)Gd(7)Co(2)) at the L(3)/L(2)-edges of Fe, Co, and Ni. The achieved ferromagnetic resonance sensitivity is about 0.1 monolayers/square root(Hz). The obtained results are interpreted in the framework of a conductivity tensor based formalism. The factors limiting the sensitivity as well as different approaches for the x-ray detection of ferromagnetic resonance are discussed.

  20. Magnetic Untwisting in Most Solar X-Ray Jets

    Science.gov (United States)

    Moore, Ronald; Sterling, Alphonse; Falconer, David; Robe, Dominic

    2013-01-01

    From 54 X-ray jets observed in the polar coronal holes by Hinode's X-Ray Telescope (XRT) during coverage in movies from Solar Dynamic Observatory's Atmospheric Imaging Assembly (AIA) taken in its He II 304 Å band at a cadence of 12 s, we have established a basic characteristic of solar X-ray jets: untwisting motion in the spire. In this presentation, we show the progression of few of these X-ray jets in XRT images and track their untwisting in AIA He II images. From their structure displayed in their XRT movies, 19 jets were evidently standard jets made by interchange reconnection of the magnetic-arcade base with ambient open field, 32 were evidently blowout jets made by blowout eruption of the base arcade, and 3 were of ambiguous form. As was anticipated from the >10,000 km span of the base arcade in most polar X-ray jets and from the disparity of standard jets and blowout jets in their magnetic production, few of the standard X-ray jets (3 of 19) but nearly all of the blowout X-ray jets (29 of 32) carried enough cool (T is approximately 105 K) plasma to be seen in their He II movies. In the 32 X-ray jets that showed a cool component, the He II movies show 10-100 km/s untwisting motions about the axis of the spire in all 3 standard jets and in 26 of the 29 blowout jets. Evidently, the open magnetic field in nearly all blowout X-ray jets and probably in most standard X-ray jets carries transient twist. This twist apparently relaxes by propagating out along the open field as a torsional wave. High-resolution spectrograms and Dopplergrams have shown that most Type-II spicules have torsional motions of 10-30 km/s. Our observation of similar torsional motion in X-ray jets strengthens the case for Type-II spicules being made in the same way as X-ray jets, by blowout eruption of a twisted magnetic arcade in the spicule base and/or by interchange reconnection of the twisted base arcade with the ambient open field. This work was funded by NASA's Heliophysics Division

  1. X-ray magnetic diffraction of ferromagnets with synchrotron radiation

    CERN Document Server

    Ito, M

    2002-01-01

    X-ray magnetic diffraction experiment of ferromagnets that utilizes elliptically polarized synchrotron radiation is presented. First we have reviewed shortly historical backgrounds and theoretical aspects of the experiment. We have presented how the magnetic form factors are measured and are separated into the spin-moment component and the orbital-moment component in this experiment. Peculiar features of the polarization factor of this experiment have been explained. We have introduced two examples of the experiment. One is the measurement of the spin-magnetic form factor of SmAl sub 2 with white X-rays from a bending magnet at the Photon Factory. The other is the measurement of the orbital-magnetic form factor of Holmium Iron Garnets with monochromatic X-rays from an undulator at the SPring-8. Finally we summarize the article and show some future prospects of this experiment. (author)

  2. X-ray scattering study of the interplay between magnetism and structure in CeSb

    DEFF Research Database (Denmark)

    McMorrow, Desmond Francis; Lussier, J.-G.; Lebech, Bente

    1997-01-01

    The chemical and magnetic structures of CeSb have been investigated using high-resolution x-ray scattering techniques. Experiments performed in the non-resonant regime (x-ray energy of E = 9.4 keV) showed that when the sample was cooled below its Neel temperature of T-N approximate to 16.5 K, peaks...... appeared with commensurate wave vectors q. From their polarization and wave-vector dependence, the peaks are deduced to arise mainly from a periodic lattice distortion. In the resonant regime, when the x-ray energy was tuned to the L absorption edges of Ce, weak, resonantly enhanced magnetic scattering...... of the magnetic structure of CeSb....

  3. Magnetic x-ray dichroism in ultrathin epitaxial films

    Energy Technology Data Exchange (ETDEWEB)

    Tobin, J.G.; Goodman, K.W. [Lawrence Berkeley National Lab., CA (United States); Cummins, T.R. [Univ. of Missouri, Rolla, MO (United States)] [and others

    1997-04-01

    The authors have used Magnetic X-ray Linear Dichroism (MXLD) and Magnetic X-ray Circular Dichroism (MXCD) to study the magnetic properties of epitaxial overlayers in an elementally specific fashion. Both MXLD and MXCD Photoelectron Spectroscopy were performed in a high resolution mode at the Spectromicroscopy Facility of the ALS. Circular Polarization was obtained via the utilization of a novel phase retarder (soft x-ray quarter wave plate) based upon transmission through a multilayer film. The samples were low temperature Fe overlayers, magnetic alloy films of NiFe and CoNi, and Gd grown on Y. The authors results include a direct comparison of high resolution angle resolved Photoelectron Spectroscopy performed in MXLD and MXCD modes as well as structural studies with photoelectron diffraction.

  4. Polarization of resonantly excited X-ray lines

    Science.gov (United States)

    Shah, Chintan; Amaro, Pedro; Steinbrügge, René; Bernitt, Sven; Fritzsche, Stephan; Surzhykov, Andrey; Crespo Lopez-Urrutia, José R.; Tashenov, Stanislav

    2017-08-01

    For a wide range of temperatures, resonantly captured electrons with energies below the excitation threshold are the strongest source of X-ray line excitation in hot plasmas containing highly charged Fe ions. The angular distribution and polarization of X-rays emitted due to these processes were experimentally studied using an electron beam ion trap. The electron-ion collision energy was scanned over the KLL dielectronic, trielectronic, and quadruelectronic recombination resonances of Fe18+..24+ and Kr28+..34+ with an exemplary resolution of ~6 eV. The angular distribution of induced X-ray fluorescence was measured along and perpendicular to the electron beam propagation direction [1]. Subsequently, the polarization of X-ray fluorescence was also measured using a novel Compton polarimeter [2, 3].The experimental data reveal the alignment of the populated excited states and exhibit a high sensitivity to the relativistic Breit interaction [2, 4]. We observed that most of the transitions lead to polarization, including hitherto-neglected trielectronic and quadruelectronic recombination channels. Furthermore, these channels dominate the polarization of the prominent Kα X-rays emitted by hot anisotropic plasmas in a wide temperature range. The present experimental results comprehensively benchmark full-order atomic calculations carried out with the FAC [5] and RATIP [6] codes. We conclude that accurate polarization diagnostics of hot anisotropic plasmas, e.~g., of solar flares and active galactic nuclei, and laboratory fusion plasmas of tokamaks can only be obtained under the premise of careful inclusion of relativistic effects and higher-order resonances which were often neglected in previous works [1]. The present experiments also demonstrate the suitability of the applied technique for accurate directional diagnostics of electron or ion beams in hot plasmas [7].[1] C. Shah et al., Phys. Rev. E 93, 061201 (R) (2016)[2] C. Shah et al., Phys. Rev. A 92, 042702 (2015

  5. X-RAY EMISSION FROM MAGNETIC MASSIVE STARS

    Energy Technology Data Exchange (ETDEWEB)

    Nazé, Yaël [GAPHE, Département AGO, Université de Liège, Allée du 6 Août 17, Bat. B5C, B-4000 Liège (Belgium); Petit, Véronique [Department of Physics and Space Sciences, Florida Institute of Technology, Melbourne, FL 32901 (United States); Rinbrand, Melanie; Owocki, Stan [Department of Physics and Astronomy, University of Delaware, Bartol Research Institute, Newark, DE 19716 (United States); Cohen, David [Department of Physics and Astronomy, Swarthmore College, Swarthmore, PA 19081 (United States); Ud-Doula, Asif [Penn State Worthington Scranton, Dunmore, PA 18512 (United States); Wade, Gregg A., E-mail: naze@astro.ulg.ac.be [Department of Physics, Royal Military College of Canada, PO Box 17000, Station Forces, Kingston, ON K7K 4B4 (Canada)

    2014-11-01

    Magnetically confined winds of early-type stars are expected to be sources of bright and hard X-rays. To clarify the systematics of the observed X-ray properties, we have analyzed a large series of Chandra and XMM-Newton observations, corresponding to all available exposures of known massive magnetic stars (over 100 exposures covering ∼60% of stars compiled in the catalog of Petit et al.). We show that the X-ray luminosity is strongly correlated with the stellar wind mass-loss rate, with a power-law form that is slightly steeper than linear for the majority of the less luminous, lower- M-dot B stars and flattens for the more luminous, higher- M-dot O stars. As the winds are radiatively driven, these scalings can be equivalently written as relations with the bolometric luminosity. The observed X-ray luminosities, and their trend with mass-loss rates, are well reproduced by new MHD models, although a few overluminous stars (mostly rapidly rotating objects) exist. No relation is found between other X-ray properties (plasma temperature, absorption) and stellar or magnetic parameters, contrary to expectations (e.g., higher temperature for stronger mass-loss rate). This suggests that the main driver for the plasma properties is different from the main determinant of the X-ray luminosity. Finally, variations of the X-ray hardnesses and luminosities, in phase with the stellar rotation period, are detected for some objects and they suggest that some temperature stratification exists in massive stars' magnetospheres.

  6. X-rays and magnetism: a review of program in magnetic studies with polarized soft x-rays

    Science.gov (United States)

    Fischer, Peter; Ohldag, Hendrik

    2015-09-01

    Magnetism is among the most active and attractive areas in modern solid state physics because of intriguing phenomena interesting to fundamental research and a manifold of technological applications. State-of-the-art synthesis of advanced magnetic materials, e.g. in hybrid structures paves the way to new functionalities. To characterize modern magnetic materials and the associated magnetic phenomena, polarized x-rays have emerged as unique probes due to their specific interaction with magnetic materials. A large variety of spectroscopic and microscopic techniques have been developed to quantify in an element, valence and site-sensitive way properties of ferro-, ferri-, and antiferromagnetic systems, such as spin and orbital moments, and to image nanoscale spin textures and their dynamics with sub-ns time and almost 10 nm spatial resolution. The enormous intensity of x-rays and their degree of coherence at next generation x-ray facilities will open the fsec time window to magnetic studies addressing fundamental time scales in magnetism with nanometer spatial resolution. This review will give an introduction into contemporary topics of nanoscale magnetic materials and provide an overview of analytical spectroscopy and microscopy tools based on x-ray dichroism effects. Selected examples of current research will demonstrate the potential and future directions of these techniques.

  7. Making use of x-ray optical effects in photoelectron-, Auger electron-, and x-ray emission spectroscopies: Total reflection, standing-wave excitation, and resonant effects

    Energy Technology Data Exchange (ETDEWEB)

    Yang, S.-H. [IBM Almaden Research Center, San Jose, California 95120 (United States); Gray, A. X. [Materials Sciences Division, Lawrence Berkeley National Laboratory, Berkeley, California 94740 (United States); Department of Physics, University of California at Davis, Davis, California 95616 (United States); Stanford Institute for Materials and Energy Science, Stanford University and SLAC National Accelerator Laboratory, Menlo Park, California 94025 (United States); Kaiser, A. M. [Materials Sciences Division, Lawrence Berkeley National Laboratory, Berkeley, California 94740 (United States); Department of Physics, University of California at Davis, Davis, California 95616 (United States); Peter Grunberg Institute, PGI-6, Forschungszentrum Juelich, 52425 Juelich (Germany); Mun, B. S. [Advanced Light Source, Lawrence Berkeley National Laboratory, Berkeley, California 94720 (United States); Department of Applied Physics, Hanyang University, Ansan, Gyeonggi 426-791 (Korea, Republic of); Sell, B. C. [Materials Sciences Division, Lawrence Berkeley National Laboratory, Berkeley, California 94740 (United States); Department of Physics, University of California at Davis, Davis, California 95616 (United States); Department of Physics, Otterbein College, Westerville, Ohio 43081 (United States); Kortright, J. B. [Materials Sciences Division, Lawrence Berkeley National Laboratory, Berkeley, California 94740 (United States); Fadley, C. S. [Materials Sciences Division, Lawrence Berkeley National Laboratory, Berkeley, California 94740 (United States); Department of Physics, University of California at Davis, Davis, California 95616 (United States)

    2013-02-21

    We present a general theoretical methodology and related open-access computer program for carrying out the calculation of photoelectron, Auger electron, and x-ray emission intensities in the presence of several x-ray optical effects, including total reflection at grazing incidence, excitation with standing-waves produced by reflection from synthetic multilayers and at core-level resonance conditions, and the use of variable polarization to produce magnetic circular dichroism. Calculations illustrating all of these effects are presented, including in some cases comparisons to experimental results. Sample types include both semi-infinite flat surfaces and arbitrary multilayer configurations, with interdiffusion/roughness at their interfaces. These x-ray optical effects can significantly alter observed photoelectron, Auger, and x-ray intensities, and in fact lead to several generally useful techniques for enhancing surface and buried-layer sensitivity, including layer-resolved densities of states and depth profiles of element-specific magnetization. The computer program used in this study should thus be useful for a broad range of studies in which x-ray optical effects are involved or are to be exploited in next-generation surface and interface studies of nanoscale systems.

  8. Hard X-ray properties of magnetic cataclysmic variables

    CERN Document Server

    Scaringi, S; Norton, A J; Knigge, C; Hill, A B; Clark, D J; Dean, A J; McBride, V A; Barlow, E J; Bassani, L; Bazzano, A; Fiocchi, M; Landi, R

    2009-01-01

    Hard X-ray surveys have proven remarkably efficient in detecting intermediate polars and asynchronous polars, two of the rarest type of cataclysmic variable (CV). Here we present a global study of hard X-ray selected intermediate polars and asynchronous polars, focusing particularly on the link between hard X-ray properties and spin/orbital periods. To this end, we first construct a new sample of these objects by cross-correlating candidate sources detected in INTEGRAL/IBIS observations against catalogues of known CVs. We find 23 cataclysmic variable matches, and also present an additional 9 (of which 3 are definite) likely magnetic cataclysmic variables (mCVs) identified by others through optical follow-ups of IBIS detections. We also include in our analysis hard X-ray observations from Swift/BAT and SUZAKU/HXD in order to make our study more complete. We find that most hard X-ray detected mCVs have P_{spin}/P_{orb}<0.1 above the period gap. In this respect we also point out the very low number of detecte...

  9. In situ small-angle x-ray and nuclear resonant scattering study of the evolution of structural and magnetic properties of an Fe thin film on MgO (001)

    Science.gov (United States)

    Sharma, Gagan; Gupta, Ajay; Gupta, Mukul; Schlage, Kai; Wille, H.-C.

    2015-12-01

    Growth of magnetron sputtered Fe films on clean single crystalline MgO (001) substrate has been studied using in situ grazing incidence small angle x-ray scattering (GISAXS) and grazing incidence nuclear resonant scattering (GINRS) measurements. While GISAXS provides information about morphological changes, GINRS provides information about structural and magnetic properties, thus making it possible to correlate the evolution of magnetic properties with that of morphology and structure of the film. The film exhibits a Volmer-Weber type growth, with percolation transition occurring around 2 nm film thickness. Presence of a finite quadrupole splitting, as seen in GINRS measurements, suggests a significant distortion from cubic symmetry up to a film thickness of 3.5 nm, which can be attributed to hybridization between Fe 3 d and O 2 p orbitals at the interface as well as in-plane tensile strain induced as a result of coalescence of islands. Initially Fe islands exhibit superparamagnetic relaxation, while finite magnetic moment appears upon formation of macroscopic percolation islands. The film exhibits a weak perpendicular magnetic anisotropy (PMA), which vanishes concurrently with disappearance of structural distortion, suggesting that the observed PMA at least partly originates from inherent strain in the film. No presence of any known oxide of Fe was detected at the interface. More precise information about topological and magnetic structure of the interfaces between Fe and MgO layers is obtained using combined x-ray reflectivity and nuclear resonance reflectivity measurements on a 57Fe/MgO multilayer. Measurements show that about two monolayers of Fe at the interface have a reduced hyperfine field, providing evidence for hybridization with O atoms, as predicted by theory.

  10. Logical operations with single x-ray photons via dynamically-controlled nuclear resonances.

    Science.gov (United States)

    Gunst, Jonas; Keitel, Christoph H; Pálffy, Adriana

    2016-04-27

    Photonic qubits lie at the heart of quantum information technology, often encoding information in their polarization state. So far, only low-frequency optical and infrared photons have been employed as flying qubits, as the resources that are at present easiest to control. With their essentially different way of interacting with matter, x-ray qubits would bear however relevant advantages: they are extremely robust, penetrate deep through materials, and can be focused down to few-nm waveguides, allowing unprecedented miniaturization. Also, x-rays are resonant to nuclear transitions, which are very well isolated from the environment and present long coherence times. Here, we show theoretically that x-ray polarization qubits can be dynamically controlled by nuclear Mössbauer resonances. The control knob is played by nuclear hyperfine magnetic fields, that allow via fast rotations precise processing of single x-ray quanta polarization. With such rotations, single-qubit and binary logical operations such as a destructive C-NOT gate can be implemented.

  11. Multifunctional Fe3O4/TaO(x) core/shell nanoparticles for simultaneous magnetic resonance imaging and X-ray computed tomography.

    Science.gov (United States)

    Lee, Nohyun; Cho, Hye Rim; Oh, Myoung Hwan; Lee, Soo Hong; Kim, Kangmin; Kim, Byung Hyo; Shin, Kwangsoo; Ahn, Tae-Young; Choi, Jin Woo; Kim, Young-Woon; Choi, Seung Hong; Hyeon, Taeghwan

    2012-06-27

    Multimodal imaging is highly desirable for accurate diagnosis because it can provide complementary information from each imaging modality. In this study, a sol-gel reaction of tantalum(V) ethoxide in a microemulsion containing Fe(3)O(4) nanoparticles (NPs) was used to synthesize multifunctional Fe(3)O(4)/TaO(x) core/shell NPs, which were biocompatible and exhibited a prolonged circulation time. When the NPs were intravenously injected, the tumor-associated vessel was observed using computed tomography (CT), and magnetic resonance imaging (MRI) revealed the high and low vascular regions of the tumor.

  12. Comparison of 3.0 T magnetic resonance imaging and X-ray mammography in the measurement of ductal carcinoma in situ: A comparison with histopathology

    Energy Technology Data Exchange (ETDEWEB)

    Pickles, Martin D., E-mail: m.pickles@hull.ac.uk [Centre for Magnetic Resonance Investigations, Hull York Medical School at University of Hull, Hull Royal Infirmary, Anlaby Road, Hull, HU3 2JZ (United Kingdom); Gibbs, Peter [Centre for Magnetic Resonance Investigations, Hull York Medical School at University of Hull, Hull Royal Infirmary, Anlaby Road, Hull, HU3 2JZ (United Kingdom); Hubbard, Anne; Rahman, Ayesha; Wieczorek, Joanna [Breast Care Unit, Hull & East Yorkshire Hospitals NHS Trust, Castle Hill Hospital, Castle Road, Cottingham, HU16 5JQ (United Kingdom); Turnbull, Lindsay W. [Centre for Magnetic Resonance Investigations, Hull York Medical School at University of Hull, Hull Royal Infirmary, Anlaby Road, Hull, HU3 2JZ (United Kingdom)

    2015-04-15

    Highlights: •Accuracy of X-ray mammography and MRI were assesses against histopathology results. •The highest level of agreement was noted between MRI and histopathology. •MRI provides a more accurate estimation of DCIS size than X-ray mammography. •MRI's superior size assessment was also noted for clinically relevant subdivisions. -- Abstract: Purpose: To determine if MRI data obtained at 3.0 T can more accurately report the size of DCIS as compared to radiographic mammography, as a whole cohort and when subdivided by lesion characteristics. Methods: Thirty-nine participants underwent X-ray mammography and MRI prior to breast surgery for DCIS. Longest diameter (LD) measurements were recorded for each imaging modality and compared to histopathological LD via a logarithmic transformed Bland–Altman agreement plot methodology resulting in dimensionless mean difference and 95% limits of agreement (LoA). Results: Data from 39 patients with a median age of 55 years (range 38–78 years) underwent analysis. Mastectomy was undertaken in 21 cases, while breast conserving surgery was performed in 18 subjects. Histopathological analysis revealed one low grade, nine intermediate grade, and 21 high grade lesions. The mean ± standard deviation LD measurements for histopathology, X-ray mammography and MRI were 50.6 ± 34.2 mm, 30.7 ± 23.1 mm and 49.6 ± 26.8 mm respectively. Bland–Altman agreement plot analysis for the whole cohort revealed not only a smaller logarithmic mean difference between MRI and histopathology (0.086), but also narrower 95% LoA (−0.941 to 1.113) compared with X-ray mammography and histopathology (mean difference −0.658, 95% LoA −3.503 to 2.187). When the level of agreement was assessed between clinically relevant subgroups additional significant differences were noted based on grade, hormonal receptor status, invasion, necrosis, mircocalcifications and growth pattern. Conclusion: MRI provides a more accurate estimation of DCIS size

  13. Resonant Compton Upscattering Models of Magnetar Hard X-ray Emission and Polarization

    Science.gov (United States)

    Baring, Matthew G.; Wadiasingh, Zorawar; Gonthier, Peter L.; Kust Harding, Alice

    2017-08-01

    Non-thermal quiescent X-ray emission extending between 10 keV and around 150 keV has been seen in about 10 magnetars by RXTE, INTEGRAL, Suzaku and Fermi-GBM. For inner magnetospheric models of such hard X-ray signals, resonant Compton upscattering is anticipated to be the most efficient process for generating the continuum radiation. This is because the scattering becomes resonant at the cyclotron frequency, and the effective cross section exceeds the classical Thomson value by over two orders of magnitude. We present angle-dependent hard X-ray upscattering model spectra for uncooled monoenergetic relativistic electrons injected in inner regions of pulsar magnetospheres. These spectra are integrated over closed field lines and obtained for different observing perspectives. The spectral cut-off energies are critically dependent on the observer viewing angles and electron Lorentz factor. We find that electrons with energies less than around 15 MeV will emit most of their radiation below 250 keV, consistent with the observed turnovers in magnetar hard X-ray tails. Moreover, electrons of higher energy still emit most of the radiation below around 1 MeV, except for quasi-equatorial emission locales for select pulses phases. In such cases, attenuation mechanisms such as pair creation will be prolific, thereby making it difficult to observe signals extending into the Fermi-LAT band. Our spectral computations use new state-of-the-art, spin-dependent formalism for the QED Compton scattering cross section in strong magnetic fields. The emission exhibits strong polarization above around 30 keV that is anticipated to be dependent on pulse phase, thereby defining science agendas for future hard X-ray polarimeters.

  14. Toward broad-band x-ray detected ferromagnetic resonance in longitudinal geometry

    Energy Technology Data Exchange (ETDEWEB)

    Ollefs, K. [Fakultät für Physik, Universität Duisburg-Essen, Lotharstr. 1, 47057 Duisburg (Germany); European Synchrotron Radiation Facility (ESRF), CS 40220, 38043 Grenoble Cedex (France); Meckenstock, R.; Spoddig, D.; Römer, F. M.; Hassel, Ch.; Schöppner, Ch.; Farle, M. [Fakultät für Physik, Universität Duisburg-Essen, Lotharstr. 1, 47057 Duisburg (Germany); Ney, V.; Ney, A., E-mail: andreas.ney@jku.at [Fakultät für Physik, Universität Duisburg-Essen, Lotharstr. 1, 47057 Duisburg (Germany); Institut für Halbleiter-und Festkörperphysik, Johannes Kepler Universität, Altenberger Str. 69, 4040 Linz (Austria)

    2015-06-14

    An ultrahigh-vacuum-compatible setup for broad-band X-ray detected ferromagnetic resonance (XFMR) in longitudinal geometry is introduced which relies on a low-power, continuous-wave excitation of the ferromagnetic sample. A simultaneous detection of the conventional ferromagnetic resonance via measuring the reflected microwave power and the XFMR signal of the X-ray absorption is possible. First experiments on the Fe and Co L{sub 3}-edges of a permalloy film covered with Co nanostripes as well as the Fe and Ni K-edges of a permalloy film are presented and discussed. Two different XFMR signals are found, one of which is independent of the photon energy and therefore does not provide element-selective information. The other much weaker signal is element-selective, and the dynamic magnetic properties could be detected for Fe and Co separately. The dependence of the latter XFMR signal on the photon helicity of the synchrotron light is found to be distinct from the usual x-ray magnetic circular dichroism effect.

  15. Diagnosis of initial changes in patients suffering from rheumatoid arthritis. Two years follow up control with a low-field magnetic resonance scanner, 3-phase bone scintigraphy and conventional X-ray

    Energy Technology Data Exchange (ETDEWEB)

    Hoepfner, S. [Abt. fuer Diagnostische Radiologie, Klinikum der Justus-Liebig-Univ. Giessen (Germany); Treitl, M.; Becker-Gaab, C.; Krolak, C. [Inst. fuer Klinische Radiologie, Klinikum der Ludwig-Maximilians-Univ. Muenchen (Germany); Weiss, M.; Tiling, R. [Klinik und Poliklinik fuer Nuklearmedizin, Klinikum der Ludwig-Maximilians-Univ. Muenchen (Germany)

    2004-12-01

    Besides conventional X-ray, in the diagnostic work up of initial changes in patients suffering from rheumatoid arthritis (RA), 3-phase bone scintigraphy (3P-Sz) is as well established as magnetic resonance imaging (MRI). The aim of this study was to compare the diagnostic value of a newly developed low field MRI with proven methods such as conventional X-ray and 3P-Sz. Patients, methods: 42 patients were studied using a one day's protocol with 3P-Sz, MRI, and X-ray of the hands with yearly follow up examinations. Images were visually assessed by two blinded nuclear medicine physicians and radiologists and classified as RA-typical and non-RA-typical changes. All methods were compared to the summarised findings interpreted by a rheumatologist in consideration of the Ritchie articular index as gold-standard. Results: 24/42 patients presented with clinical symptoms of initial changes by rheumatoid arthritis. Conventional X-ray revealed in 20/24 patients within the correct diagnosis in the study period. On the other hand 3P-Sz and low field MRI concordantly showed all 24 patients with initial changes due to RA. Time of detection showed variations with a tendency to later findings by conventional X-ray. Conclusions: In the diagnostic work up of initial changes conventional X-ray should be the first choice in imaging. Our findings suggest that MRI represents an equally sensitive method for the diagnosis of initial changes due to RA in the region of the hands as compared to the 3P-Sz. The limitation of the low field MRI is the small field of view, so we prefer 3P-Sz or high field MRI in the diagnosis of patients with suspected RA. (orig.) [German] In der Initialdiagnostik bei rheumatoider Arthritis (RA) werden neben der Projektionsradiographie (PR) auch die Magnetresonanztomographie (MRT) und die 3-Phasen-Skelettszintigraphie (3P-SZ) eingesetzt. Ziel dieser Studie war es, bei Patienten mit Verdacht auf RA die Wertigkeit der PR, der 3P-SZ und der MRT anhand von

  16. Anti-Stokes resonant x-ray Raman scattering for atom specific and excited state selective dynamics

    Science.gov (United States)

    Kunnus, Kristjan; Josefsson, Ida; Rajkovic, Ivan; Schreck, Simon; Quevedo, Wilson; Beye, Martin; Grübel, Sebastian; Scholz, Mirko; Nordlund, Dennis; Zhang, Wenkai; Hartsock, Robert W.; Gaffney, Kelly J.; Schlotter, William F.; Turner, Joshua J.; Kennedy, Brian; Hennies, Franz; Techert, Simone; Wernet, Philippe; Odelius, Michael; Föhlisch, Alexander

    2016-10-01

    Ultrafast electronic and structural dynamics of matter govern rate and selectivity of chemical reactions, as well as phase transitions and efficient switching in functional materials. Since x-rays determine electronic and structural properties with elemental, chemical, orbital and magnetic selectivity, short pulse x-ray sources have become central enablers of ultrafast science. Despite of these strengths, ultrafast x-rays have been poor at picking up excited state moieties from the unexcited ones. With time-resolved anti-Stokes resonant x-ray Raman scattering (AS-RXRS) performed at the LCLS, and ab initio theory we establish background free excited state selectivity in addition to the elemental, chemical, orbital and magnetic selectivity of x-rays. This unparalleled selectivity extracts low concentration excited state species along the pathway of photo induced ligand exchange of Fe(CO)5 in ethanol. Conceptually a full theoretical treatment of all accessible insights to excited state dynamics with AS-RXRS with transform-limited x-ray pulses is given—which will be covered experimentally by upcoming transform-limited x-ray sources.

  17. Soft X-ray measurements in magnetic fusion plasma physics

    Science.gov (United States)

    Botrugno, A.; Gabellieri, L.; Mazon, D.; Pacella, D.; Romano, A.

    2010-11-01

    Soft X-ray diagnostic systems and their successful application in the field of magnetic fusion plasma physics are discussed. Radiation with wavelength in the region of Soft X-Ray (1-30 keV) is largely produced by high temperature plasmas, carrying important information on many processes during a plasma discharge. Soft X-ray diagnostics are largely used in various fusion devices all over the world. These diagnostic systems are able to obtain information on electron temperature, electron density, impurity transport, Magneto Hydro Dynamic instabilities. We will discuss the SXR diagnostic installed on FTU in Frascati (Italy) and on Tore Supra in Cadarache (France), with special emphasis on diagnostic performances. Moreover, we will discuss the two different inversion methods for tomographic reconstruction used in Frascati and in Cadarache, the first one is relied on a guessed topology of iso-emissivity surfaces, the second one on regularization techniques, like minimum Fisher or maximum entropy. Finally, a new and very fast 2D imaging system with energy discrimination and high time resolution will be summarized as an alternative approach of SXR detection system.

  18. Reproducibility and accuracy of body composition assessments in mice by dual energy x-ray absorptiometry and time domain nuclear magnetic resonance.

    Science.gov (United States)

    Halldorsdottir, Solveig; Carmody, Jill; Boozer, Carol N; Leduc, Charles A; Leibel, Rudolph L

    2009-01-01

    OBJECTIVE: To assess the accuracy and reproducibility of dual-energy absorptiometry (DXA; PIXImus(™)) and time domain nuclear magnetic resonance (TD-NMR; Bruker Optics) for the measurement of body composition of lean and obese mice. SUBJECTS AND MEASUREMENTS: Thirty lean and obese mice (body weight range 19-67 g) were studied. Coefficients of variation for repeated (x 4) DXA and NMR scans of mice were calculated to assess reproducibility. Accuracy was assessed by comparing DXA and NMR results of ten mice to chemical carcass analyses. Accuracy of the respective techniques was also assessed by comparing DXA and NMR results obtained with ground meat samples to chemical analyses. Repeated scans of 10-25 gram samples were performed to test the sensitivity of the DXA and NMR methods to variation in sample mass. RESULTS: In mice, DXA and NMR reproducibility measures were similar for fat tissue mass (FTM) (DXA coefficient of variation [CV]=2.3%; and NMR CV=2.8%) (P=0.47), while reproducibility of lean tissue mass (LTM) estimates were better for DXA (1.0%) than NMR (2.2%) (advantages compared to DXA, such as speed of measurement and the ability to scan unanesthetized animals.

  19. Registration of planar bioluminescence to magnetic resonance and x-ray computed tomography images as a platform for the development of bioluminescence tomography reconstruction algorithms.

    Science.gov (United States)

    Beattie, Bradley J; Klose, Alexander D; Le, Carl H; Longo, Valerie A; Dobrenkov, Konstantine; Vider, Jelena; Koutcher, Jason A; Blasberg, Ronald G

    2009-01-01

    The procedures we propose make possible the mapping of two-dimensional (2-D) bioluminescence image (BLI) data onto a skin surface derived from a three-dimensional (3-D) anatomical modality [magnetic resonance (MR) or computed tomography (CT)] dataset. This mapping allows anatomical information to be incorporated into bioluminescence tomography (BLT) reconstruction procedures and, when applied using sources visible to both optical and anatomical modalities, can be used to evaluate the accuracy of those reconstructions. Our procedures, based on immobilization of the animal and a priori determined fixed projective transforms, should be more robust and accurate than previously described efforts, which rely on a poorly constrained retrospectively determined warping of the 3-D anatomical information. Experiments conducted to measure the accuracy of the proposed registration procedure found it to have a mean error of 0.36+/-0.23 mm. Additional experiments highlight some of the confounds that are often overlooked in the BLT reconstruction process, and for two of these confounds, simple corrections are proposed.

  20. X-ray edge singularity in resonant inelastic x-ray scattering (RIXS)

    Science.gov (United States)

    Markiewicz, Robert; Rehr, John; Bansil, Arun

    2013-03-01

    We develop a lattice model based on the theory of Mahan, Noziéres, and de Dominicis for x-ray absorption to explore the effect of the core hole on the RIXS cross section. The dominant part of the spectrum can be described in terms of the dynamic structure function S (q , ω) dressed by matrix element effects, but there is also a weak background associated with multi-electron-hole pair excitations. The model reproduces the decomposition of the RIXS spectrum into well- and poorly-screened components. An edge singularity arises at the threshold of both components. Fairly large lattice sizes are required to describe the continuum limit. Supported by DOE Grant DE-FG02-07ER46352 and facilitated by the DOE CMCSN, under grant number DE-SC0007091.

  1. X-ray and neutron scattering studies of magnetic critical fluctuations in holmium

    Energy Technology Data Exchange (ETDEWEB)

    Thurston, T.R.; Helgesen, G.; Gibbs, D.; Shirane, G. [Brookhaven National Lab., Upton, NY (United States); Hill, J.P. [Brookhaven National Lab., Upton, NY (United States)]|[Massachusetts Inst. of Tech., Cambridge, MA (United States). Dept. of Physics; Gaulin, B.D. [Brookhaven National Lab., Upton, NY (United States)]|[McMaster Univ., Hamilton, ON (Canada). Dept. of Physics

    1993-04-01

    We describe measurements of the magnetic critical fluctuations of holmium by x-ray scattering techniques. The x-ray results are compared to those obtained in neutron scattering experiments performed on the same sample.

  2. X-ray and neutron scattering studies of magnetic critical fluctuations in holmium

    Energy Technology Data Exchange (ETDEWEB)

    Thurston, T.R.; Helgesen, G.; Gibbs, D.; Shirane, G. (Brookhaven National Lab., Upton, NY (United States)); Hill, J.P. (Brookhaven National Lab., Upton, NY (United States) Massachusetts Inst. of Tech., Cambridge, MA (United States). Dept. of Physics); Gaulin, B.D. (Brookhaven National Lab., Upton, NY (United States) McMaster Univ., Hamilton, ON (Canada). Dept. of Physics)

    1993-01-01

    We describe measurements of the magnetic critical fluctuations of holmium by x-ray scattering techniques. The x-ray results are compared to those obtained in neutron scattering experiments performed on the same sample.

  3. Quantitative x-ray magnetic circular dichroism mapping with high spatial resolution full-field magnetic transmission soft x-ray spectro-microscopy

    Energy Technology Data Exchange (ETDEWEB)

    Robertson, MacCallum J. [Center for X-ray Optics, Lawrence Berkeley National Laboratory, Berkeley, California 94720 (United States); Physics Department, University of California, Berkeley, California 94720 (United States); Agostino, Christopher J. [Physics Department, University of California, Berkeley, California 94720 (United States); National Center for Electron Microscopy, Lawrence Berkeley National Laboratory, Berkeley, California 94720 (United States); N' Diaye, Alpha T. [Advanced Light Source, Lawrence Berkeley National Laboratory, Berkeley, California 94720 (United States); Chen, Gong [National Center for Electron Microscopy, Lawrence Berkeley National Laboratory, Berkeley, California 94720 (United States); Im, Mi-Young [Center for X-ray Optics, Lawrence Berkeley National Laboratory, Berkeley, California 94720 (United States); Department of Emerging Materials Science, Daegu Gyeongbuk Institute of Science and Technology, Daegu 711-873 (Korea, Republic of); Fischer, Peter, E-mail: PJFischer@lbl.gov [Center for X-ray Optics, Lawrence Berkeley National Laboratory, Berkeley, California 94720 (United States); Physics Department, University of California, Santa Cruz, California 94056 (United States)

    2015-05-07

    The spectroscopic analysis of X-ray magnetic circular dichroism (XMCD), which serves as strong and element-specific magnetic contrast in full-field magnetic transmission soft x-ray microscopy, is shown to provide information on the local distribution of spin (S) and orbital (L) magnetic moments down to a spatial resolution of 25 nm limited by the x-ray optics used in the x-ray microscope. The spatially resolved L/S ratio observed in a multilayered (Co 0.3 nm/Pt 0.5 nm) × 30 thin film exhibiting a strong perpendicular magnetic anisotropy decreases significantly in the vicinity of domain walls, indicating a non-uniform spin configuration in the vertical profile of a domain wall across the thin film. Quantitative XMCD mapping with x-ray spectro-microscopy will become an important characterization tool for systems with topological or engineered magnetization inhomogeneities.

  4. X-ray resonant exchange scattering of rare-earth nickel borocarbides

    Energy Technology Data Exchange (ETDEWEB)

    Detlefs, C.

    1997-10-08

    The purpose of this thesis is to investigate the systematics of the microscopic magnetic order within a series of isostructural compounds and, at the same, to develop the relatively young experimental method of x-ray resonant exchange scattering (XRES). In this thesis, the author presents XRES studies of several rare-earth nickel borocarbides, RNi{sub 2}B{sub 2}C. He shows that XRES, similar to the neutron techniques, allows the determination of the orientation of the magnetic moment by measuring the Q-dependence of the scattered intensity of magnetic Bragg reflections. As samples in this study, he chose the recently discovered family of rare-earth nickel borocarbides, RNi{sub 2}B{sub 2}C, which display a wide variety of magnetic structures. Furthermore, in several of these materials, long range magnetic order coexists with superconductivity over some temperature range.

  5. Non-invasive methods for the determination of body and carcass composition in livestock: dual-energy X-ray absorptiometry, computed tomography, magnetic resonance imaging and ultrasound: invited review.

    Science.gov (United States)

    Scholz, A M; Bünger, L; Kongsro, J; Baulain, U; Mitchell, A D

    2015-07-01

    The ability to accurately measure body or carcass composition is important for performance testing, grading and finally selection or payment of meat-producing animals. Advances especially in non-invasive techniques are mainly based on the development of electronic and computer-driven methods in order to provide objective phenotypic data. The preference for a specific technique depends on the target animal species or carcass, combined with technical and practical aspects such as accuracy, reliability, cost, portability, speed, ease of use, safety and for in vivo measurements the need for fixation or sedation. The techniques rely on specific device-driven signals, which interact with tissues in the body or carcass at the atomic or molecular level, resulting in secondary or attenuated signals detected by the instruments and analyzed quantitatively. The electromagnetic signal produced by the instrument may originate from mechanical energy such as sound waves (ultrasound - US), 'photon' radiation (X-ray-computed tomography - CT, dual-energy X-ray absorptiometry - DXA) or radio frequency waves (magnetic resonance imaging - MRI). The signals detected by the corresponding instruments are processed to measure, for example, tissue depths, areas, volumes or distributions of fat, muscle (water, protein) and partly bone or bone mineral. Among the above techniques, CT is the most accurate one followed by MRI and DXA, whereas US can be used for all sizes of farm animal species even under field conditions. CT, MRI and US can provide volume data, whereas only DXA delivers immediate whole-body composition results without (2D) image manipulation. A combination of simple US and more expensive CT, MRI or DXA might be applied for farm animal selection programs in a stepwise approach.

  6. Real-time high-resolution X-ray imaging and nuclear magnetic resonance study of the hydration of pure and Na-doped C3A in the presence of sulfates

    Energy Technology Data Exchange (ETDEWEB)

    Kirchheim,, A. P.; Dal Molin, D.C.; Emwas, Abdul-Hamid; Provis, J.L.; Fischer, P.; Monteiro, P.J.M.

    2010-12-01

    This study details the differences in real-time hydration between pure tricalcium aluminate (cubic C{sub 3}A or 3CaO {center_dot} Al{sub 2}O{sub 3}) and Na-doped tricalcium aluminate (orthorhombic C{sub 3}A or Na{sub 2}Ca{sub 8}Al{sub 6}O{sub 18}), in aqueous solutions containing sulfate ions. Pure phases were synthesized in the laboratory to develop an independent benchmark for the reactions, meaning that their reactions during hydration in a simulated early age cement pore solution (saturated with respect to gypsum and lime) were able to be isolated. Because the rate of this reaction is extremely rapid, most microscopy methods are not adequate to study the early phases of the reactions in the early stages. Here, a high-resolution full-field soft X-ray imaging technique operating in the X-ray water window, combined with solution analysis by {sup 27}Al nuclear magnetic resonance (NMR) spectroscopy, was used to capture information regarding the mechanism of C{sub 3}A hydration during the early stages. There are differences in the hydration mechanism between the two types of C{sub 3}A, which are also dependent on the concentration of sulfate ions in the solution. The reactions with cubic C{sub 3}A (pure) seem to be more influenced by higher concentrations of sulfate ions, forming smaller ettringite needles at a slower pace than the orthorhombic C{sub 3}A (Na-doped) sample. The rate of release of aluminate species into the solution phase is also accelerated by Na doping.

  7. Real-time high-resolution X-ray imaging and nuclear magnetic resonance study of the hydration of pure and Na-doped C3A in the presence of sulfates

    KAUST Repository

    Kirchheim, A. P.

    2011-02-21

    This study details the differences in real-time hydration between pure tricalcium aluminate (cubic C3A or 3CaO·Al2O 3) and Na-doped tricalcium aluminate (orthorhombic C3A or Na2Ca8Al6O18), in aqueous solutions containing sulfate ions. Pure phases were synthesized in the laboratory to develop an independent benchmark for the reactions, meaning that their reactions during hydration in a simulated early age cement pore solution (saturated with respect to gypsum and lime) were able to be isolated. Because the rate of this reaction is extremely rapid, most microscopy methods are not adequate to study the early phases of the reactions in the early stages. Here, a high-resolution full-field soft X-ray imaging technique operating in the X-ray water window, combined with solution analysis by 27Al nuclear magnetic resonance (NMR) spectroscopy, was used to capture information regarding the mechanism of C3A hydration during the early stages. There are differences in the hydration mechanism between the two types of C3A, which are also dependent on the concentration of sulfate ions in the solution. The reactions with cubic C3A (pure) seem to be more influenced by higher concentrations of sulfate ions, forming smaller ettringite needles at a slower pace than the orthorhombic C3A (Na-doped) sample. The rate of release of aluminate species into the solution phase is also accelerated by Na doping. © 2011 American Chemical Society.

  8. Characterization of tetra-aryl benzene isomers by using preparative gas chromatography with mass spectrometry, nuclear magnetic resonance spectroscopy, and X-ray crystallographic methods.

    Science.gov (United States)

    Rühle, Christian P G; Niere, Julie; Morrison, Paul D; Jones, Roderick C; Caradoc-Davies, Tom; Canty, Allan J; Gardiner, Michael G; Tolhurst, Vicki-Anne; Marriott, Philip J

    2010-06-01

    The present study describes a preparative gas chromatographic (GC) approach employed to study a series of products arising from reaction of phenylacetylene with para-substituted aryl-iodides under Sonogashira catalysis conditions. GC analysis resolves the isomers from each reaction; however, it cannot provide structural details (their MS data are virtually identical). Since classical liquid chromatography cannot resolve the isomers, preparative-scale GC is the only practical approach to provide further spectroscopic characterization of the isomers. The products are well separated by GC so a single thick-film capillary column is adequate for this case, with operation up to approximately +300 degrees C. By collection of 50+ repeat injections, sufficient material could be isolated for (1)H NMR spectral analysis of the isomers, and for one isomer (isomer I) of a number of analogous related catalytic reaction mixtures, X-ray crystal structure determination enabled complete structural elucidation (absolute configuration) of the substitution pattern of the structure of this isomer. This confirmed isomer I to be the 2-para-aryl-substituted 1,3,5-triphenylbenzene product in all cases. (1)H NMR spectra of isomer I products generally had similar patterns but differed markedly from the second major isomer product (isomer II).

  9. Monolayer to interdigitated partial bilayer smectic C transition in thiophene-based spacer mesogens: X-ray diffraction and (13)C nuclear magnetic resonance studies.

    Science.gov (United States)

    Kesava Reddy, M; Varathan, E; Lobo, Nitin P; Roy, Arun; Narasimhaswamy, T; Ramanathan, K V

    2015-10-06

    Mesophase organization of molecules built with thiophene at the center and linked via flexible spacers to rigid side arm core units and terminal alkoxy chains has been investigated. Thirty homologues realized by varying the span of the spacers as well as the length of the terminal chains have been studied. In addition to the enantiotropic nematic phase observed for all the mesogens, the increase of the spacer as well as the terminal chain lengths resulted in the smectic C phase. The molecular organization in the smectic phase as investigated by temperature dependent X-ray diffraction measurements revealed an interesting behavior that depended on the length of the spacer vis-a-vis the length of the terminal chain. Thus, a tilted interdigitated partial bilayer organization was observed for molecules with a shorter spacer length, while a tilted monolayer arrangement was observed for those with a longer spacer length. High-resolution solid state (13)C NMR studies carried out for representative mesogens indicated a U-shape for all the molecules, indicating that intermolecular interactions and molecular dynamics rather than molecular shape are responsible for the observed behavior. Models for the mesophase organization have been considered and the results understood in terms of segregation of incompatible parts of the mesogens combined with steric frustration leading to the observed lamellar order.

  10. Physics of orbital degree of freedom - resonant X-ray scattering for observation of orbital ordering

    CERN Document Server

    Hirota, K

    2003-01-01

    Orbital degree of freedom plays very important roles in electric and magnetic properties in strongly correlated electron systems. The method for measurement of orbital ordering, however, has been limited so far. Recently it has been pointed out that the resonant X-ray scattering (RXS) technique is a very powerful tool to observe the ordering. In ths paper, the principle of RXS and the recent development are described after the general introduction of orbital degree of freedom. Finally the future in orbital physics will be discussed. (author)

  11. Local-spin-selective x-ray absorption and x-ray magnetic circular dichroism of MnP

    NARCIS (Netherlands)

    Groot, F.M.F. de; Pizzini, S.; Fontaine, A.; Hämäläinen, K.; Kao, C.C.; Hastings, J.B.

    1995-01-01

    The local-spin-selective X-ray absorption spectrum and the magnetic circular dichroism (MCD) spectrum are measured at the manganese K edge of MnP. A comparison of the two techniques makes it possible to determine the energy dependence of the Fano factor. It is found that the Fano factor is -4% at

  12. Time-resolved X-ray transmission microscopy on magnetic microstructures; Zeitaufloesende Roentgentransmissionsmikroskopie an magnetischen Mikrostrukturen

    Energy Technology Data Exchange (ETDEWEB)

    Puzic, Aleksandar

    2007-10-23

    Three excitation schemes were designed for stroboscopic imaging of magnetization dynamics with time-resolved magnetic transmission X-ray microscopy (TR-MTXM). These techniques were implemented into two types of X-ray microscopes, namely the imaging transmission X-ray microscope (ITXM) and the scanning transmission X-ray microscope (STXM), both installed at the electron storage ring of the Advanced Light Source in Berkeley, USA. Circular diffraction gratings (Fresnel zone plates) used in both microscopes as focusing and imaging elements presently allow for lateral resolution down to 30 nm. Magnetic imaging is performed by using the X-ray magnetic circular dichroism (XMCD) as element specific contrast mechanism. The developed methods have been successfully applied to the experimental investigation of magnetization dynamics in ferromagnetic microstructures. A temporal resolution well below 100 ps was achieved. A conventional pump-probe technique was implemented first. The dynamic response of the magnetization excited by a broadband pulsed magnetic field was imaged spatially resolved using focused X-ray flashes. As a complementary method, the spatially resolved ferromagnetic resonance (SR-FMR) technique was developed for experimental study of magnetization dynamics in the frequency domain. As a third excitation mode, the burst excitation was implemented. The performance and efficiency of the developed methods have been demonstrated by imaging the local magnetization dynamics in laterally patterned ferromagnetic thin-film elements and three-layer stacks. The existence of multiple eigenmodes in the excitation spectra of ferromagnetic microstructures has been verified by using the pump-probe technique. Magnetostatic spin waves were selectively excited and detected with a time resolution of 50 ps using the SR-FMR technique. Thorough analysis of 20 in most cases independently prepared samples has verified that vortices which exhibit a low-amplitude switching of their core

  13. Direct surface magnetometry with photoemission magnetic x-ray dichroism

    Energy Technology Data Exchange (ETDEWEB)

    Tobin, J.G.; Goodman, K.W. [Lawrence Berkeley National Lab., CA (United States); Schumann, F.O. [Pennsylvania State Univ., University Park, PA (United States)] [and others

    1997-04-01

    Element specific surface magnetometry remains a central goal of synchrotron radiation based studies of nanomagnetic structures. One appealing possibility is the combination of x-ray absorption dichroism measurements and the theoretical framework provided by the {open_quotes}sum rules.{close_quotes} Unfortunately, sum rule analysis are hampered by several limitations including delocalization of the final state, multi-electronic phenomena and the presence of surface dipoles. An alternative experiment, Magnetic X-Ray Dichroism in Photoelectron Spectroscopy, holds out promise based upon its elemental specificity, surface sensitivity and high resolution. Computational simulations by Tamura et al. demonstrated the relationship between exchange and spin orbit splittings and experimental data of linear and circular dichroisms. Now the authors have developed an analytical framework which allows for the direct extraction of core level exchange splittings from circular and linear dichroic photoemission data. By extending a model initially proposed by Venus, it is possible to show a linear relation between normalized dichroism peaks in the experimental data and the underlying exchange splitting. Since it is reasonable to expect that exchange splittings and magnetic moments track together, this measurement thus becomes a powerful new tool for direct surface magnetometry, without recourse to time consuming and difficult spectral simulations. The theoretical derivation will be supported by high resolution linear and circular dichroism data collected at the Spectromicroscopy Facility of the Advanced Light Source.

  14. Magnetic soft x-ray microscopy-imaging fast spin dynamics inmagnetic nanostructures

    Energy Technology Data Exchange (ETDEWEB)

    Fischer, Peter; Kim, Dong-Hyun; Mesler, Brooke L.; Chao, Weilun; Sakdinawat, Anne E.; Anderson, Erik H.

    2007-06-01

    Magnetic soft X-ray microscopy combines 15nm spatial resolution with 70ps time resolution and elemental sensitivity. Fresnel zone plates are used as X-ray optics and X-ray magnetic circular dichroism serves as magnetic contrast mechanism. Thus scientifically interesting and technologically relevant low dimensional nanomagnetic systems can be imaged at fundamental length and ultrafast time scales in a unique way. Studies include magnetization reversal in magnetic multilayers, nanopatterned systems, vortex dynamics in nanoelements and spin current induced phenomena.

  15. Performance of Magnetic Penetration Thermometers for X-Ray Astronomy

    Science.gov (United States)

    Nagler, P. C.; Adams, J. S.; Balvin, M. A.; Bandler, S. R.; Denis, K. L.; Hsieh, W. T.; Kelly, D. P.; Porst, J. P.; Sadleir, J. E.; Seidel, G. M.; hide

    2012-01-01

    The ideal X-ray camera for astrophysics would have more than a million pixels and provide an energy resolution of better than leV FWHM for energies up to 10 keY. We have microfabricated and characterized thin-film magnetic penetration thermometers (MPTs) that show great promise towards meeting these capabilities. MPTs operate in similar fashion to metallic magnetic calorimeters (MMCs), except that a superconducting sensor takes the place of a paramagnetic sensor and it is the temperature dependence of the superconductor's diamagnetic response that provides the temperature sensitivity. We present a description of the design and performance of our prototype thin-film MPTs with MoAu bilayer sensors, which have demonstrated an energy resolution of approx 2 eV FWHM at 1.5 keY and 4.3 eV FWHM at 5.9 keY.

  16. Performance of Magnetic Penetration Thermometers for X-Ray Astronomy

    Science.gov (United States)

    Nagler, P. C.; Adams, J. S.; Balvin, M. A.; Bandler, S. R.; Denis, K. L.; Hsieh, W. T.; Kelly, D. P.; Porst, J. P.; Sadleir, J. E.; Seidel, G. M.; Smith, S. J.; Stevenson, T. R.

    2012-01-01

    The ideal X-ray camera for astrophysics would have more than a million pixels and provide an energy resolution of better than leV FWHM for energies up to 10 keY. We have microfabricated and characterized thin-film magnetic penetration thermometers (MPTs) that show great promise towards meeting these capabilities. MPTs operate in similar fashion to metallic magnetic calorimeters (MMCs), except that a superconducting sensor takes the place of a paramagnetic sensor and it is the temperature dependence of the superconductor's diamagnetic response that provides the temperature sensitivity. We present a description of the design and performance of our prototype thin-film MPTs with MoAu bilayer sensors, which have demonstrated an energy resolution of approx 2 eV FWHM at 1.5 keY and 4.3 eV FWHM at 5.9 keY.

  17. Magnetic nanoparticles studied by small angle X-ray scattering

    Energy Technology Data Exchange (ETDEWEB)

    Oliveira, Cristiano Luis Pinto [Universidade de Sao Paulo (IF/USP), SP (Brazil). Inst. de Fisica. Grupo de Fluidos Complexos; Antonel, Soledad; Negri, Martin [Universidad de Buenos Aires (UBA) (Argentina). Facultad de Ciencias Exactas y Naturales. Dept. de Quimica Inorganica, Analitica y Quimica Fisica

    2011-07-01

    nanoparticles are very interesting because they exhibit magnetic (ferromagnetic) and electrical properties in the same material. Then, the nickel nanoparticles could be used for the development of electroelastic materials. In this case, the electrical conductivity of the material can be strongly dependent on the applied magnetic field, for example the case of nickel metal nanoparticles dispersed in a polymer, resulting in an anisotropic material with combined piezomagnetic and piezoelectric properties. In order to investigate the structural characteristics of cobalt-iron oxides and nickel nanoparticles, powder samples of those magnetic materials were studied by Small-Angle X-Ray Scattering. As will be shown, from the analysis and modeling of the scattering data, structural information could be obtained, enabling a detailed description of the structural properties of the studied samples which could be directly correlated to the magnetic properties. (author)

  18. Gd3+ complex-modified NaLuF4-based upconversion nanophosphors for trimodality imaging of NIR-to-NIR upconversion luminescence, X-Ray computed tomography and magnetic resonance.

    Science.gov (United States)

    Xia, Ao; Chen, Min; Gao, Yuan; Wu, Dongmei; Feng, Wei; Li, Fuyou

    2012-07-01

    Multimodality molecular imaging has recently attracted much attention, because it can take advantage of individual imaging modalities by fusing together information from several molecular imaging techniques. Herein, we report a multifunctional lanthanide-based nanoparticle for near-infrared to near-infrared (NIR-to-NIR) upconversion luminescence (UCL), X-ray computed tomography (CT) and T(1)-enhanced magnetic resonance (MR) trimodality in-vivo imaging. By careful selection of the lanthanide elements, core-shell structured lanthanide-based nanoparticles, NaLuF(4):Yb(3+),Tm(3+)@SiO(2)-GdDTPA nanoparticles (UCNP@SiO(2)-GdDTPA) have been designed and synthesized. We also prove that the application of UCNP@SiO(2)-GdDTPA for NIR-to-NIR UCL, CT and MRI multi-modality in-vivo imaging can be established successfully. In addition, the biological toxicity of UCNP@SiO(2)-GdDTPA is evaluated by the methyl thiazolyl tetrazolium (MTT) assay and histological analysis of viscera sections. Copyright © 2012 Elsevier Ltd. All rights reserved.

  19. Comparison of X-ray powder diffraction and solid-state nuclear magnetic resonance in estimating crystalline fraction of tacrolimus in sustained-release amorphous solid dispersion and development of discriminating dissolution method.

    Science.gov (United States)

    Rahman, Ziyaur; Bykadi, Srikant; Siddiqui, Akhtar; Khan, Mansoor A

    2015-05-01

    The focus of present investigation was to explore X-ray powder diffraction (XRPD) and solid-state nuclear magnetic resonance (ssNMR) techniques for amorphous and crystalline tacrolimus quantification in the sustained-release amorphous solid dispersion (ASD), and to propose discriminating dissolution method that can detect crystalline drug. The ASD and crystalline physical mixture was mixed in various proportions to make sample matrices containing 0%-100% crystalline-amorphous tacrolimus. Partial-least-square regression and principle component regression were applied to the spectral data. Dissolution of the ASD in the US FDA recommended dissolution medium with and without surfactant was performed. R(2) > 0.99 and slope was close to one for all the models. Root-mean-square of prediction, standard error of prediction, and bias were higher in ssNMR-based models when compared with XRPD data models. Dissolution of the ASD decreased with an increase in the crystalline tacrolimus in the formulations. Furthermore, detection of crystalline tacrolimus in the ASD was progressively masked with an increase in the surfactant level in the dissolution medium. XRPD and ssNMR can be used equally to quantitate the crystalline and amorphous fraction of tacrolimus in the ASD with good accuracy; however, ssNMR data collection time is excessively long, and minimum surfactant level in the dissolution medium maximizes detection of crystalline reversion in the formulation.

  20. Resonant x-ray scattering in 3d-transition-metal oxides: Anisotropy and charge orderings

    Science.gov (United States)

    Subías, G.; García, J.; Blasco, J.; Herrero-Martín, J.; Sánchez, M. C.

    2009-11-01

    The structural, magnetic and electronic properties of transition metal oxides reflect in atomic charge, spin and orbital degrees of freedom. Resonant x-ray scattering (RXS) allows us to perform an accurate investigation of all these electronic degrees. RXS combines high-Q resolution x-ray diffraction with the properties of the resonance providing information similar to that obtained by atomic spectroscopy (element selectivity and a large enhancement of scattering amplitude for this particular element and sensitivity to the symmetry of the electronic levels through the multipole electric transitions). Since electronic states are coupled to the local symmetry, RXS reveals the occurrence of symmetry breaking effects such as lattice distortions, onset of electronic orbital ordering or ordering of electronic charge distributions. We shall discuss the strength of RXS at the K absorption edge of 3d transition-metal oxides by describing various applications in the observation of local anisotropy and charge disproportionation. Examples of these resonant effects are (I) charge ordering transitions in manganites, Fe3O4 and ferrites and (II) forbidden reflections and anisotropy in Mn3+ perovskites, spinel ferrites and cobalt oxides. In all the studied cases, the electronic (charge and/or anisotropy) orderings are determined by the structural distortions.

  1. A new X-ray detector for magnetic circular dichroism experiments

    CERN Document Server

    Bateman, J E; Dudzik, E; Laan, G V D; Lipp, J D; Smith, A D; Stephenson, R

    2001-01-01

    X-ray magnetic circular dichroism (XMCD) studies of magnetic 3d transition metal samples require the recording of high quality absorption scans in high magnetic fields using circularly polarised soft X-rays of energies in the range 0.5-1 keV. A Gas Microstrip Detector is described which permits the option of using the X-ray fluorescence signal instead of the usual electron yield signal.

  2. Sapphire hard X-ray Fabry-Perot resonators for synchrotron experiments.

    Science.gov (United States)

    Tsai, Yi Wei; Wu, Yu Hsin; Chang, Ying Yi; Liu, Wen Chung; Liu, Hong Lin; Chu, Chia Hong; Chen, Pei Chi; Lin, Pao Te; Fu, Chien Chung; Chang, Shih Lin

    2016-05-01

    Hard X-ray Fabry-Perot resonators (FPRs) made from sapphire crystals were constructed and characterized. The FPRs consisted of two crystal plates, part of a monolithic crystal structure of Al2O3, acting as a pair of mirrors, for the backward reflection (0 0 0 30) of hard X-rays at 14.3147 keV. The dimensional accuracy during manufacturing and the defect density in the crystal in relation to the resonance efficiency of sapphire FPRs were analyzed from a theoretical standpoint based on X-ray cavity resonance and measurements using scanning electron microscopic and X-ray topographic techniques for crystal defects. Well defined resonance spectra of sapphire FPRs were successfully obtained, and were comparable with the theoretical predictions.

  3. Soft X-Ray Magnetic Imaging of Focused Ion Beam Lithographically Patterned Fe Thin Films

    Energy Technology Data Exchange (ETDEWEB)

    Cook, Paul J.; Shen, Tichan H.; Grundy, PhilJ.; Im, Mi Young; Fischer, Peter; Morton, Simon A.; Kilcoyne, Arthur D.L.

    2008-11-09

    We illustrate the potential of modifying the magnetic behavior and structural properties of ferromagnetic thin films using focused ion beam 'direct-write' lithography. Patterns inspired by the split-ring resonators often used as components in meta-materials were defined upon 15 nm Fe films using a 30 keV Ga{sup +} focused ion beam at a dose of 2 x 10{sup 16} ions cm{sup -2}. Structural, chemical and magnetic changes to the Fe were studied using transmission soft X-ray microscopy at the ALS, Berkeley CA. X-ray absorption spectra showed a 23% reduction in the thickness of the film in the Ga irradiated areas, but no change to the chemical environment of Fe was evident. X-ray images of the magnetic reversal process show domain wall pinning around the implanted areas, resulting in an overall increase in the coercivity of the film. Transmission electron microscopy showed significant grain growth in the implanted regions.

  4. Generation of linearly polarized resonant transition radiation X-ray beam

    Energy Technology Data Exchange (ETDEWEB)

    Yajima, Kazuaki; Awata, Takaaki; Ikeda, Mitsuharu; Ikeda, Kenichi; Yogo, Akifumi; Itoh, Akio; Imanishi, Nobutsugu [Kyoto Univ. (Japan). Dept. of Nuclear Engineering

    2000-03-01

    We have proposed a method to generate almost linearly polarized resonant transition radiation X rays by using a rectangular slit placed on an electron beam axis. Our calculation predicted that the linearity is 93.5% for the resonant transition radiation X-ray beam extracted through a slit of 0.5 mrad long and 0.2 mrad wide in case of 1-GeV electron beam irradiating a 7.5-{mu}m thick Kapton foil stack. (author)

  5. Soft x-ray ptychography studies of nanoscale magnetic and structural correlations in thin SmCo{sub 5} films

    Energy Technology Data Exchange (ETDEWEB)

    Shi, X. [Advanced Light Source, Lawrence Berkeley National Laboratory, Berkeley, California 94720 (United States); Department of Physics, University of Oregon, Eugene, Oregon 97401 (United States); Fischer, P. [Materials Sciences Division, Lawrence Berkeley National Laboratory, Berkeley, California 94720 (United States); Department of Physics, University of California, Santa Cruz, California 94056 (United States); Neu, V.; Elefant, D. [IFW Dresden, Institute for Metallic Materials, Helmholtzstr. 20, D-01069 Dresden (Germany); Lee, J. C. T.; Kevan, S. D., E-mail: SDKevan@lbl.gov [Advanced Light Source, Lawrence Berkeley National Laboratory, Berkeley, California 94720 (United States); Department of Physics, University of Oregon, Eugene, Oregon 97401 (United States); Materials Sciences Division, Lawrence Berkeley National Laboratory, Berkeley, California 94720 (United States); Shapiro, D. A.; Farmand, M.; Tyliszczak, T.; Marchesini, S.; Roy, S. [Advanced Light Source, Lawrence Berkeley National Laboratory, Berkeley, California 94720 (United States); Shiu, H.-W. [Advanced Light Source, Lawrence Berkeley National Laboratory, Berkeley, California 94720 (United States); National Synchrotron Radiation Research Center (NSRRC), 101 Hsin-Ann Road, Hsinchu Science Park, Hsinchu 30076, Taiwan (China)

    2016-02-29

    High spatial resolution magnetic x-ray spectromicroscopy at x-ray photon energies near the cobalt L{sub 3} resonance was applied to probe an amorphous 50 nm thin SmCo{sub 5} film prepared by off-axis pulsed laser deposition onto an x-ray transparent 200 nm thin Si{sub 3}N{sub 4} membrane. Alternating gradient magnetometry shows a strong in-plane anisotropy and an only weak perpendicular magnetic anisotropy, which is confirmed by magnetic transmission soft x-ray microscopy images showing over a field of view of 10 μm a primarily stripe-like domain pattern but with local labyrinth-like domains. Soft x-ray ptychography in amplitude and phase contrast was used to identify and characterize local magnetic and structural features over a field of view of 1 μm with a spatial resolution of about 10 nm. There, the magnetic labyrinth domain patterns are accompanied by nanoscale structural inclusions that are primarily located in close proximity to the magnetic domain walls. Our analysis suggests that these inclusions are nanocrystalline Sm{sub 2}Co{sub 17} phases with nominally in-plane magnetic anisotropy.

  6. X-ray studies of neutron stars and their magnetic fields

    Science.gov (United States)

    MAKISHIMA, Kazuo

    2016-01-01

    Utilizing results obtained over the past quarter century mainly with Japanese X-ray astronomy satellites, a review is given to some aspects of neutron stars (NSs), with a particular emphasis on the magnetic fields (MFs) of mass-accreting NSs and magnetars. Measurements of electron cyclotron resonance features in binary X-ray pulsars, using the Ginga and Suzaku observatories, clarified that their surface MFs are concentrated in a narrow range of (1–7) × 108 T. Extensive studies of magnetars with Suzaku reinforced their nature as neutron stars with truly strong MFs, and revealed several important clues to their formation, evolution, and physical states. Taking all these results into account, a discussion is made on the origin and evolution of these strong MFs. One possible scenario is that the MF of NSs is a manifestation of some fundamental physics, e.g., neutron spin alignment or chirality violation, and the MF makes transitions from strong to weak states. PMID:27169348

  7. X-ray studies of neutron stars and their magnetic fields.

    Science.gov (United States)

    Makishima, Kazuo

    2016-01-01

    Utilizing results obtained over the past quarter century mainly with Japanese X-ray astronomy satellites, a review is given to some aspects of neutron stars (NSs), with a particular emphasis on the magnetic fields (MFs) of mass-accreting NSs and magnetars. Measurements of electron cyclotron resonance features in binary X-ray pulsars, using the Ginga and Suzaku observatories, clarified that their surface MFs are concentrated in a narrow range of (1-7) × 10(8) T. Extensive studies of magnetars with Suzaku reinforced their nature as neutron stars with truly strong MFs, and revealed several important clues to their formation, evolution, and physical states. Taking all these results into account, a discussion is made on the origin and evolution of these strong MFs. One possible scenario is that the MF of NSs is a manifestation of some fundamental physics, e.g., neutron spin alignment or chirality violation, and the MF makes transitions from strong to weak states.

  8. Shimming with permanent magnets for the x-ray detector in a hybrid x-ray/ MR system.

    Science.gov (United States)

    Wen, Zhifei; Fahrig, Rebecca; Williams, Scott T; Pelc, Norbert J

    2008-09-01

    In this x-ray/MR hybrid system an x-ray flat panel detector is placed under the patient cradle, close to the MR volume of interest (VOI), where the magnetic field strength is approximately 0.5 T. Immersed in this strong field, several electronic components inside the detector become magnetized and create an additional magnetic field that is superimposed on the original field of the MR scanner. Even after linear shimming, the field homogeneity of the MR scanner remains disrupted by the detector. The authors characterize the field due to the detector with the field of two magnetic dipoles and further show that two sets of permanent magnets (NdFeB) can withstand the main magnetic field and compensate for the nonlinear components of the additional field. The ideal number of magnets and their locations are calculated based on a field map measured with the detector in place. Experimental results demonstrate great promise for this technique, which may be useful in many settings where devices with magnetic components need to be placed inside or close to an MR scanner.

  9. Electrostatic focal spot correction for x-ray tubes operating in strong magnetic fields.

    Science.gov (United States)

    Lillaney, Prasheel; Shin, Mihye; Hinshaw, Waldo; Fahrig, Rebecca

    2014-11-01

    A close proximity hybrid x-ray/magnetic resonance (XMR) imaging system offers several critical advantages over current XMR system installations that have large separation distances (∼5 m) between the imaging fields of view. The two imaging systems can be placed in close proximity to each other if an x-ray tube can be designed to be immune to the magnetic fringe fields outside of the MR bore. One of the major obstacles to robust x-ray tube design is correcting for the effects of the MR fringe field on the x-ray tube focal spot. Any fringe field component orthogonal to the x-ray tube electric field leads to electron drift altering the path of the electron trajectories. The method proposed in this study to correct for the electron drift utilizes an external electric field in the direction of the drift. The electric field is created using two electrodes that are positioned adjacent to the cathode. These electrodes are biased with positive and negative potential differences relative to the cathode. The design of the focusing cup assembly is constrained primarily by the strength of the MR fringe field and high voltage standoff distances between the anode, cathode, and the bias electrodes. From these constraints, a focusing cup design suitable for the close proximity XMR system geometry is derived, and a finite element model of this focusing cup geometry is simulated to demonstrate efficacy. A Monte Carlo simulation is performed to determine any effects of the modified focusing cup design on the output x-ray energy spectrum. An orthogonal fringe field magnitude of 65 mT can be compensated for using bias voltages of +15 and -20 kV. These bias voltages are not sufficient to completely correct for larger orthogonal field magnitudes. Using active shielding coils in combination with the bias electrodes provides complete correction at an orthogonal field magnitude of 88.1 mT. Introducing small fields (rotation of the x-ray tube by 30° toward the MR bore increases the

  10. The high-field magnet endstation for X-ray magnetic dichroism experiments at ESRF soft X-ray beamline ID32

    Science.gov (United States)

    Kummer, K.; Fondacaro, A.; Jimenez, E.; Velez-Fort, E.; Amorese, A.; Aspbury, M.; Yakhou-Harris, F.; van der Linden, P.; Brookes, N. B.

    2016-01-01

    A new high-field magnet endstation for X-ray magnetic dichroism experiments has been installed and commissioned at the ESRF soft X-ray beamline ID32. The magnet consists of two split-pairs of superconducting coils which can generate up to 9 T along the beam and up to 4 T orthogonal to the beam. It is connected to a cluster of ultra-high-vacuum chambers that offer a comprehensive set of surface preparation and characterization techniques. The endstation and the beam properties have been designed to provide optimum experimental conditions for X-ray magnetic linear and circular dichroism experiments in the soft X-ray range between 400 and 1600 eV photon energy. User operation started in November 2014. PMID:26917134

  11. Improving the spatial resolution of a soft X-ray Charge Coupled Device used for Resonant Inelastic X-ray Scattering

    OpenAIRE

    Soman, M. R.; Hall, D. J. (David John); Tutt, J. H.; Murray, N. J.; Holland, A. D.; Schmitt, T.; Raabe, J.; Schmitt, B.

    2011-01-01

    The Super Advanced X-ray Emission Spectrometer (SAXES) at the Advanced Resonant Scattering (ADRESS) beamline of the Swiss Light Source is a high-resolution X-ray spectrometer used as an end station for Resonant Inelastic X-ray Scattering from 400 eV to 1600 eV. Through the dispersion of photons across a CCD, the energy of scattered photons may be determined by their detected spatial position. The limiting factor of the energy resolution is currently the spatial resolution achieved with the CC...

  12. Study of magnetic transitions in samarium using X-ray scattering

    CERN Document Server

    Stunault, A

    2001-01-01

    Extensive use has been made of synchrotron X-ray magnetic and charge scattering to study the temperature dependence of long range magnetic order in a samarium film and of the related magnetostrictive effects. Resonant magnetic scattering is shell selective and the behavior of the 4f and 5d electrons could be studied separately through the magnetic phase transitions, with the photon energy tuned close to the samarium L/sub 3/ absorption edge. Simultaneously, lattice distortions at the magnetic phase transitions have been evidenced by the study of strong charge reflections with sufficiently high resolution. Weak charge reflections are also present and are interpreted in terms of deviations of the hexagonal samarium planes from equidistant positions in the c-direction. (7 refs).

  13. Imaging nanoscale magnetic structures with polarized soft x-ray photons

    Energy Technology Data Exchange (ETDEWEB)

    Fischer, P.; Im, M.-Y.

    2010-01-18

    Imaging nanoscale magnetic structures and their fast dynamics is scientifically interesting and technologically of highest relevance. The combination of circularly polarized soft X-ray photons which provide a strong X-ray magnetic circular dichroism effect at characteristic X-ray absorption edges, with a high resolution soft X-ray microscope utilizing Fresnel zone plate optics allows to study in a unique way the stochastical behavior in the magnetization reversal process of thin films and the ultrafast dynamics of magnetic vortices and domain walls in confined ferromagnetic structures. Future sources of fsec short and high intense soft X-ray photon pulses hold the promise of magnetic imaging down to fundamental magnetic length and time scales.

  14. An analysis of imaging characteristics of X-ray, computed tomography and magnetic resonance imaging of intraosseous lipoma%骨内脂肪瘤的X线、CT和MRI影像学特点分析

    Institute of Scientific and Technical Information of China (English)

    李春爱; 栾贻新; 程晓光; 李相龙

    2014-01-01

    Objective To investigate the imaging characteristics of X-ray, computed tomography ( CT ) and magnetic resonance imaging ( MRI ) of intraosseous lipoma and to improve the accuracy of diagnosis and differential diagnosis.Methods The imaging characteristics of X-ray, CT and MRI in 38 cases of intraosseous lipoma conifrmed by percutaneous puncture biopsy and pathological test were analyzed retrospectively, which was compared with pathological outcomes.Results Intraosseous lipoma was noticed in the calcaneus (n=11 ), in the femur (n=8 ), in the tibia (n=5 ), in the ilium (n=6 ), in the humerus (n=6 ), in the radius ( n=1 ) and in the talus (n=1 ) respectively. There were 38 cases of single cystic type in all. Based on the X-ray and CT, calciifcation was found in 11 cases, bone crest in 19 cases, double sclerotic band in 4 cases, sclerotic border in 21 cases and bone expansion in 16 cases. Lipo density could be determined by CT in all the cases. The CT value was -40HU - -133HU. The MRI showed there was fat component in all the cases. Among them, cyst formation was detected in 9 cases, and inhomogeneous signal in 20 cases. According to Milgram’s stage, 4 cases were at stage I, 4 cases at stage II and 30 cases at stage III. Conclusions The X-ray and CT can show the lesion site, morphology, calcification, bone crest, sclerotic border, bone expansion and with or without boundary. The MRI can make clear fat component, fat necrosis, cyst formation, myxoid change, inlfammation, range and border of the lesion. The X-ray, CT and MRI relfect imaging characteristics of intraosseous lipoma from different aspects.%目的:探讨骨内脂肪瘤(intraosseouslipoma,IOL)的X线、CT和MRI的影像学特点及诊断价值,提高诊断及鉴别诊断的准确性。方法回顾性分析38例经皮穿刺活检和手术病理证实的IOLX线、CT和MRI影像学特点,并与病理结果进行对照。结果38例IOL发生部位分别为:跟骨11例,股骨8例,胫骨5

  15. Free-electron laser based resonant inelastic X-ray scattering on molecules and liquids

    Energy Technology Data Exchange (ETDEWEB)

    Kunnus, Kristjan, E-mail: kkunnus@stanford.edu [Institute for Methods and Instrumentation for Synchrotron Radiation Research, Helmholtz-Zentrum Berlin GmbH, Albert-Einstein-Str. 15, 12489 Berlin (Germany); Institut für Physik und Astronomie, Universität Potsdam, Karl-Liebknecht-Str. 24/25, 14476 Potsdam (Germany); Schreck, Simon; Föhlisch, Alexander [Institute for Methods and Instrumentation for Synchrotron Radiation Research, Helmholtz-Zentrum Berlin GmbH, Albert-Einstein-Str. 15, 12489 Berlin (Germany); Institut für Physik und Astronomie, Universität Potsdam, Karl-Liebknecht-Str. 24/25, 14476 Potsdam (Germany)

    2015-10-15

    Highlights: • Femtosecond time-resolved RIXS can be used to follow charge, spin and structural dynamics of dilute solute molecules in solution. • Ultrashort X-ray pulses allow probing of highly radiation sensitive states of matter. • Nonlinear X-ray probes provide an enhanced selectivity and sensitivity as well as a path to control radiation damage and increase the photon yields in RIXS experiments. - Abstract: The unprecedented beam properties of free-electron laser based X-ray sources enable novel resonant inelastic X-ray scattering (RIXS) experiments. Femtosecond time-resolved RIXS can be used to follow charge, spin and structural dynamics of dilute solute molecules in solution. Ultrashort X-ray pulses allow probing of highly radiation sensitive states of matter such as the metastable phase of supercooled liquid water. Nonlinear X-ray probes like amplified spontaneous emission and stimulated resonant X-ray scattering provide an enhanced selectivity and sensitivity as well as a path to control radiation damage and increase the photon yields in RIXS experiments.

  16. X-Ray Polarization Optics and Coherent Nuclear Resonance Scattering Using Synchrotron Radiation.

    Science.gov (United States)

    Shastri, Sarvjit Devdat

    1995-01-01

    Two projects, both involving X-ray scattering with synchrotron radiation, are presented in this dissertation. (1) A system of diffracting perfect crystals for the generation of variable, elliptically polarized X-rays was tested at the Cornell High Energy Synchrotron Source under the conditions of a standard undulator source. The phase retarding optical component was a 4-bounce, Ge(220) Bragg reflection channel -cut crystal. The full polarization state (density matrix) of the output beam, including the circular polarization purity P_3, was determined using the multiple-beam Bragg diffraction technique with a GaAs crystal polarimeter and was found to agree with calculations. In addition to measuring the optics' efficiency, the ability to scan the system in energy, while frequently reversing the circular helicity, was demonstrated at the vicinity of the Fe K-edge at 7.1 keV. The setup was applied to a circular magnetic X-ray dichroism measurement. (2) The time distribution of delayed photons from resonant forward scattering of 14.4 keV synchrotron radiation pulses by ^{57}Fe nuclei was investigated over the temperature range from 9 K to just above the Curie point at 1043 K, with particular attention to precise measurements of the Lamb-Mossbauer factor f_{LM } ~ e^{- } , whose change was determined from its influence on the "speed-up" of coherent decay. Apart from its importance in Mossbauer effect studies, knowing the temperature dependence of f_{LM} can be valuable for studies of lattice dynamics and structural phase transitions. The change in the nuclear hyperfine splitting was also measured. The synchrotron technique has precision-enhancing advantages over conventional Mossbauer spectroscopy methods employing radioactive sources because dealing with source effects and absolute intensity measurements is eliminated. The results also straightforwardly illustrate an interesting principle concerning the temperature dependence of scattering --that for "slow" resonance

  17. Resonant X-Ray Scattering and the jeff=1/2 Electronic Ground State in Iridate Perovskites

    DEFF Research Database (Denmark)

    Sala, M. Moretti; Boseggia, S.; McMorrow, Desmond Francis

    2014-01-01

    The resonant x-ray scattering (magnetic elastic, RXMS, and inelastic, RIXS) of Ir4+ at the L-2,L-3 edges relevant to spin-orbit Mott insulators A(n+1) Ir(n)O3(n+1) (A = Sr, Ba, etc.) are calculated using a single-ion model which treats the spin-orbit and tetragonal crystal-field terms on an equal...

  18. Topological X-Rays Revisited

    Science.gov (United States)

    Lynch, Mark

    2012-01-01

    We continue our study of topological X-rays begun in Lynch ["Topological X-rays and MRI's," iJMEST 33(3) (2002), pp. 389-392]. We modify our definition of a topological magnetic resonance imaging and give an affirmative answer to the question posed there: Can we identify a closed set in a box by defining X-rays to probe the interior and without…

  19. High-resolution soft X-ray beamline ADRESS at the Swiss Light Source for resonant inelastic X-ray scattering and angle-resolved photoelectron spectroscopies

    Energy Technology Data Exchange (ETDEWEB)

    Strocov, V. N., E-mail: vladimir.strocov@psi.ch; Schmitt, T.; Flechsig, U.; Schmidt, T.; Imhof, A.; Chen, Q.; Raabe, J. [Swiss Light Source, Paul Scherrer Institut, CH-5232 Villigen-PSI (Switzerland); Betemps, R.; Zimoch, D.; Krempasky, J. [Paul Scherrer Institut, CH-5232 Villigen-PSI (Switzerland); Wang, X. [Swiss Light Source, Paul Scherrer Institut, CH-5232 Villigen-PSI (Switzerland); Institut de Physique de la Matiére Condensé, Ecole Polytechnique Fédéderale de Lausanne (Switzerland); Grioni, M. [Institut de Physique de la Matiére Condensé, Ecole Polytechnique Fédéderale de Lausanne (Switzerland); Piazzalunga, A. [Swiss Light Source, Paul Scherrer Institut, CH-5232 Villigen-PSI (Switzerland); Dipartimento di Fisica, Politecnico di Milano, Piazza Leonardo da Vinci 32, I-20133 Milano (Italy); Patthey, L. [Swiss Light Source, Paul Scherrer Institut, CH-5232 Villigen-PSI (Switzerland)

    2010-09-01

    Concepts and technical realization of the high-resolution soft X-ray beamline ADRESS at the Swiss Light Source are described. Optimization of the optical scheme for high resolution and photon flux as well as diagnostics tools and alignment strategies are discussed. The concepts and technical realisation of the high-resolution soft X-ray beamline ADRESS operating in the energy range from 300 to 1600 eV and intended for resonant inelastic X-ray scattering (RIXS) and angle-resolved photoelectron spectroscopy (ARPES) are described. The photon source is an undulator of novel fixed-gap design where longitudinal movement of permanent magnetic arrays controls not only the light polarization (including circular and 0–180° rotatable linear polarizations) but also the energy without changing the gap. The beamline optics is based on the well established scheme of plane-grating monochromator operating in collimated light. The ultimate resolving power E/ΔE is above 33000 at 1 keV photon energy. The choice of blazed versus lamellar gratings and optimization of their profile parameters is described. Owing to glancing angles on the mirrors as well as optimized groove densities and profiles of the gratings, the beamline is capable of delivering high photon flux up to 1 × 10{sup 13} photons s{sup −1} (0.01% BW){sup −1} at 1 keV. Ellipsoidal refocusing optics used for the RIXS endstation demagnifies the vertical spot size down to 4 µm, which allows slitless operation and thus maximal transmission of the high-resolution RIXS spectrometer delivering E/ΔE > 11000 at 1 keV photon energy. Apart from the beamline optics, an overview of the control system is given, the diagnostics and software tools are described, and strategies used for the optical alignment are discussed. An introduction to the concepts and instrumental realisation of the ARPES and RIXS endstations is given.

  20. Studying Nanoscale Magnetism and its Dynamics with Soft X-ray Microscopy

    Energy Technology Data Exchange (ETDEWEB)

    Mccall, Monnikue M; Fischer, Peter

    2008-05-01

    Magnetic soft X-ray microscopy allows for imaging magnetic structures at a spatial resolution down to 15nm and a time resolution in the sub-100ps regime. Inherent elemental specificity can be used to image the magnetic response of individual components such as layers in multilayered systems. This review highlights current achievements and discusses the future potential of magnetic soft X-ray microscopy at fsec X-ray sources where snapshot images of ultrafast spin dynamics with a spatial resolution below 10nm will become feasible.

  1. Probing symmetry and symmetry breaking in resonant soft-x-ray fluorescence spectra of molecules

    Energy Technology Data Exchange (ETDEWEB)

    Glans, P.; Gunnelin, K.; Guo, J. [Uppsala Univ. (Sweden)] [and others

    1997-04-01

    Conventional non-resonant soft X-ray emission brings about information about electronic structure through its symmetry and polarization selectivity, the character of which is governed by simple dipole rules. For centro-symmetric molecules with the emitting atom at the inversion center these rules lead to selective emission through the required parity change. For the more common classes of molecules which have lower symmetry or for systems with degenerate core orbitals (delocalized over identical sites), it is merely the local symmetry selectivity that provides a probe of the local atomic orbital contribution to the molecular orbital. For instance, in X-ray spectra of first row species the intensities essentially map the p-density at each particular atomic site, and, in a molecular orbital picture, the contribution of the local p-type atomic orbitals in the LCAO description of the molecular orbitals. The situation is different for resonant X-ray fluorescence spectra. Here strict parity and symmetry selectivity gives rise to a strong frequency dependence for all molecules with an element of symmetry. In addition to symmetry selectivity the strong frequency dependence of resonant X-ray emission is caused by the interplay between the shape of a narrow X-ray excitation energy function and the lifetime and vibrational broadenings of the resonantly excited core states. This interplay leads to various observable effects, such as linear dispersion, resonance narrowing and emission line (Stokes) doubling. Also from the point of view of polarization selectivity, the resonantly excited X-ray spectra are much more informative than the corresponding non-resonant spectra. Examples are presented for nitrogen, oxygen, and carbon dioxide molecules.

  2. Molecular orientation in soft matter thin films studied by resonant soft X-ray reflectivity

    Energy Technology Data Exchange (ETDEWEB)

    Mezger, Markus; Jerome, Blandine; Kortright, Jeffrey B.; Valvidares, Manuel; Gullikson, Eric; Giglia, Angelo; Mahne, Nicola; Nannarone, Stefano

    2011-01-12

    We present a technique to study depth profiles of molecular orientation in soft matter thin films with nanometer resolution. The method is based on dichroism in resonant soft X-ray reflectivity using linear s- and p-polarization. It combines the chemical sensitivity of Near-Edge X-ray Absorption Fine Structure spectroscopy to specific molecular bonds and their orientation relative to the polarization of the incident beam with the precise depth profiling capability of X-ray reflectivity. We demonstrate these capabilities on side chain liquid crystalline polymer thin films with soft X-ray reflectivity data at the carbon K edge. Optical constants of the anisotropic refractive index ellipsoid were obtained from a quantitative analysis using the Berreman formalism. For films up to 50 nm thickness we find that the degree of orientation of the long axis exhibits no depth variation and isindependent of the film thickness.

  3. ELECTRONIC CORRELATIONS IN NI 2P AND 3P MAGNETIC-X-RAY DICHROISM AND X-RAY PHOTOEMISSION OF FERROMAGNETIC NICKEL

    NARCIS (Netherlands)

    VANDERLAAN, G; THOLE, BT

    1992-01-01

    The magnetic x-ray dichroism (MXD) in x-ray absorption together with the photoemission of the Ni 2p and 3p levels in ferromagnetic nickel have been analysed using an Anderson impurity model taking into account multiplet splitting. Good agreement with experimental results was obtained for a ground

  4. Lifetime-vibrational interference effects in resonantly excited x-ray emission spectra of CO

    Energy Technology Data Exchange (ETDEWEB)

    Skytt, P.; Glans, P.; Gunnelin, K. [Uppsala Univ. (Sweden)] [and others

    1997-04-01

    The parity selection rule for resonant X-ray emission as demonstrated for O{sub 2} and N{sub 2} can be seen as an effect of interference between coherently excited degenerate localized core states. One system where the core state degeneracy is not exact but somewhat lifted was previously studied at ALS, namely the resonant X-ray emission of amino-substituted benzene (aniline). It was shown that the X-ray fluorescence spectrum resulting from excitation of the C1s at the site of the {open_quotes}aminocarbon{close_quotes} could be described in a picture separating the excitation and the emission processes, whereas the spectrum corresponding to the quasi-degenerate carbons could not. Thus, in this case it was necessary to take interference effects between the quasi-degenerate intermediate core excited states into account in order to obtain agreement between calculations and experiment. The different vibrational levels of core excited states in molecules have energy splittings which are of the same order of magnitude as the natural lifetime broadening of core excitations in the soft X-ray range. Therefore, lifetime-vibrational interference effects are likely to appear and influence the band shapes in resonant X-ray emission spectra. Lifetime-vibrational interference has been studied in non-resonant X-ray emission, and in Auger spectra. In this report the authors discuss results of selectively excited soft X-ray fluorescence spectra of molecules, where they focus on lifetime-interference effects appearing in the band shapes.

  5. Formation of X-ray emitting stationary shocks in magnetized protostellar jets

    CERN Document Server

    Ustamujic, S; Bonito, R; Miceli, M; de Castro, A I Gómez; López-Santiago, J

    2016-01-01

    X-ray observations of protostellar jets show evidence of strong shocks heating the plasma up to temperatures of a few million degrees. In some cases, the shocked features appear to be stationary. They are interpreted as shock diamonds. We aim at investigating the physics that guides the formation of X-ray emitting stationary shocks in protostellar jets, the role of the magnetic field in determining the location, stability, and detectability in X-rays of these shocks, and the physical properties of the shocked plasma. We performed a set of 2.5-dimensional magnetohydrodynamic numerical simulations modelling supersonic jets ramming into a magnetized medium and explored different configurations of the magnetic field. The model takes into account the most relevant physical effects, namely thermal conduction and radiative losses. We compared the model results with observations, via the emission measure and the X-ray luminosity synthesized from the simulations. Our model explains the formation of X-ray emitting stat...

  6. Experimental elucidation: microscopic mechanism of resonant X-ray scattering in manganite films

    CERN Document Server

    Ohsumi, H; Kiyama, T

    2003-01-01

    Resonant X-ray scattering experiments have been performed on perovskite manganite La sub 0 sub . sub 5 Sr sub 0 sub . sub 5 MnO sub 3 thin films, which are grown on three distinct perovskite with a coherent epitaxial strain and have a forced ferro-type orbital ordering of Mn 3d orbitals. Using an interference technique, we have successfully observed the resonant X-ray scattering signal from the system having the ferro-type orbital ordering and also revealed the energy scheme of Mn 4p bands. For the forced ferro-type orbital ordering system, the present results evidence that the resonant X-ray scattering signal originates from the band structure effect due to the Jahn-Teller distortion of a MnO sub 6 octahedron, and not from the Coulomb interaction between 3d and 4p electrons. (author)

  7. Resonant soft X-ray emission and X-ray absorption studies on Ga{sub 1-x}Mn{sub x}N grown by pulsed laser deposition

    Energy Technology Data Exchange (ETDEWEB)

    Krishnamurthy, Satheesh [School of Physics, Trinity College Dublin, College Green, Dublin 2 (Ireland); School of Physical Sciences, Dublin City University, Glasnevin, Dublin 9 (Ireland); Kennedy, Brian; McGee, Fintan; Venkatesan, M.; Coey, J.M.D.; Lunney, James G.; McGuinness, Cormac [School of Physics, Trinity College Dublin, College Green, Dublin 2 (Ireland); Learmonth, Timothy; Smith, Kevin E. [Department of Physilightlycs, Boston University, 590 Commonwealth Avenue, MA 02215 (United States); Schmitt, Thorsten [Swiss Light Source, Paul Scherrer Institut, 5232 Villigen PSI (Switzerland)

    2011-05-15

    In this study thin film samples of Ga{sub 1-x}Mn{sub x}N were grown by pulsed laser deposition on Al{sub 2}O{sub 3} (0001) substrates. X-ray diffraction measurements have confirmed these thin films exhibit hexagonal wurtzite structure. SQUID measurements show room temperature ferromagnetism of these dilute magnetic semiconductors (DMS). The techniques of X-ray absorption and soft X-ray emission spectroscopy at the N K-edge were used to study the changes in the unoccupied and occupied N 2p partial density of states respectively as a function of dopant concentration. These element and site specific spectroscopies allow us to characterise the electronic structure of these doped materials and reveal the influence of the Mn doping on the valence band as measured through the N 2p partial density of states. X-ray absorption measurements at the Mn L-edge confirm significant substitutional doping of Mn into Ga-sites. Finally, measurements of heavily Mn-doped films using both soft X-ray absorption and resonant soft X-ray emission at the N K edge reveal the presence of trapped molecular nitrogen. The trapped molecular nitrogen may be due to the high instantaneous deposition rate in the PLD process for these samples (copyright 2011 WILEY-VCH Verlag GmbH and Co. KGaA, Weinheim) (orig.)

  8. Discovery of extended X-ray emission around the highly magnetic RRAT J1819-1458

    NARCIS (Netherlands)

    Rea, N.; McLaughlin, M.A.; Gaensler, B.M.; Slane, P.O.; Stella, L.; Reynolds, S.P.; Burgay, M.; Israel, G.L.; Possenti, A.; Chatterjee, S.

    2009-01-01

    We report on the discovery of extended X-ray emission around the high magnetic field rotating radio transient J1819-1458. Using a 30 ks Chandra ACIS-S observation, we found significant evidence for extended X-ray emission with a peculiar shape: a compact region out to similar to 5.'' 5, and more dif

  9. Correlating properties and microstructure of YBCO thin films by magnetic X-ray microscopy

    Energy Technology Data Exchange (ETDEWEB)

    Ruoss, Stephen; Stahl, Claudia; Weigand, Markus; Schuetz, Gisela [Max-Planck-Institute for Intelligent Systems, Heisenbergstrasse 3, 70569 Stuttgart (Germany); Zahn, Patrick; Bayer, Jonas [Max-Planck-Institute for Intelligent Systems, Heisenbergstrasse 3, 70569 Stuttgart (Germany); Research Institute for Innovative Surfaces, FINO, Aalen University, Beethovenstrasse 1, 73430 Aalen (Germany); Albrecht, Joachim [Research Institute for Innovative Surfaces, FINO, Aalen University, Beethovenstrasse 1, 73430 Aalen (Germany)

    2016-07-01

    The magnetic flux distribution in high-temperature superconductors namely YBCO has been observed using a novel high-resolution technique based on the X-ray magnetic circular dichroism (XMCD). Therefore, a CoFeB layer is deposited on the superconductor which exhibits a strong XMCD-effect. X-ray absorption measurements with circular polarized radiation allows the analysis of the magnetic flux distribution in the superconductor via the soft-magnetic sensor layer [3,4]. In the total electron yield (TEY) mode of the scanning X-ray microscope (SXM) the surface structure and the magnetic domains can be imaged at the same time. Having obtained such high resolution images, the correlation of magnetic flux penetration and defect structure of YBCO thin films can be analyzed. The measurements have been performed at the scanning X-ray microscope MAXYMUS at Bessy II, HZB Berlin.

  10. Resonant Auger Destruction and Iron K-Alpha Spectra in Compact X-ray Sources

    OpenAIRE

    Liedahl, Duane A.

    2005-01-01

    We examine the effects of resonant Auger destruction in modifying the intensities and flux distributions of K-alpha spectra from iron L-shell ions. Applications include X-ray irradiated stellar winds in X-ray binaries and accretion disk atmospheres. Using detailed atomic models, we find that resonant Auger destruction is selective, in that only a subset of the emitted K-alpha lines is highly attenuated. We also show that that the local excitation conditions can have a dramatic effect on the K...

  11. In vivo body composition in autochthonous and conventional pig breeding groups by dual-energy X-ray absorptiometry and magnetic resonance imaging under special consideration of Cerdo Ibérico.

    Science.gov (United States)

    Kremer, P V; Fernández-Fígares, I; Förster, M; Scholz, A M

    2012-12-01

    The improvement of carcass quality is one of the main breeding goals in pig production. To select appropriate breeding animals, it is of major concern to exactly and reliably analyze the body composition in vivo. Therefore, the objective of the study was to examine whether the combination of dual-energy X-ray absorptiometry (DXA) and magnetic resonance imaging (MRI) offers the opportunity to reliably analyze quantitative and qualitative body composition characteristics of different pig breeding groups in vivo. In this study, a total of 77 pigs were studied by DXA and MRI at an average age of 154 days. The pigs originated from different autochthonous or conventional breeds or crossbreeds and were grouped into six breed types: Cerdo Ibérico (Ib); Duroc × Ib (Du_Ib); White Sow Lines (WSL, including German Landrace and German Large White); Hampshire/Pietrain (Pi_Ha, including Hampshire, Pietrain × Hampshire (PiHa) and Pietrain × PiHa); Pietrain/Duroc (Pi_Du, including Pietrain × Duroc (PiDu) and Pietrain × PiDu); crossbred WSL (PiDu_WSL, including Pietrain × WSL and PiDu × WSL). A whole-body scan was performed by DXA with a GE Lunar DPX-IQ in order to measure the amount and percentage of fat tissue (FM; %FM), lean tissue (LM; %LM) and bone mineral, whereas a Siemens Magnetom Open with a large body coil was used for MRI in the thorax region between 13th and 14th vertebrae in order to measure the area of the loin (LA) and the above back fat area (FA) of both body sides. A GLM procedure using SAS 9.2 was used to analyze the data. As expected, the native breed Ib followed by Du_Ib crossbreeds showed the highest %FM (27.2%, 25.0%) combined with the smallest LA (46.2 cm2, 73.6 cm2), whereas Ib had the lowest BW at an average age of 154 days. Pigs with Pi_Ha origin presented the least %FM (12.4%) and largest LA (99.5 cm2). The WSL and PiDu_WSL showed an intermediate body composition. Therefore, it could be concluded that DXA and MRI and especially their combination

  12. Hard X-ray Observations of Magnetic Cataclysmic Variables

    CERN Document Server

    Singh, K P; Mukerjee, K; Barrett, P; Schlegel, E M

    2003-01-01

    Hard X-ray light curves and spectral parameters from our analysis of X-ray data of five AM Her type systems - V2301 Oph, V1432 Aql, EP Draconis, GG Leonis, V834 Cen, and one intermediate polar - TV Col, observed using the Rossi X-ray Timing Explorer satellite are presented. A new improved ephemeris has been derived for V2301 Oph using the mid-eclipse timings. Average intensity variations, without any change of shape of the light curve or hardness ratio, are observed on timescales of a few days to a few months in V2301 Oph. V1432 Aql shows erratic variations on a timescale of a day, at least 2 sharp dips near orbital phases 0.35 and 0.5, and a total eclipse. Hard X-ray eclipses are also reported in EP Dra and GG Leo. V834 Cen shows intensity variations on yearly timescale and is found to be in a low state in 2002. In TV Col, a binary orbital modulation at 5.5h, in addition to the spin period of 1910s, is reported for the first time. Maximum spectral temperatures in Polars have been determined and used to estim...

  13. X-ray scattering studies of lanthanides magnetism

    DEFF Research Database (Denmark)

    McMorrow, D.; Bohr, Jakob; Gibbs, D.

    1999-01-01

    Interest in the applications of X-ray synchrotron radiation has grown rapidly during the last decade. At the present time, intense, ultra-bright synchrotron radiation is available on a routine basis from third-generation sources located in Europe (ESRF), North America (APS) and Japan (Spring8). T...

  14. X-ray comb generation from nuclear-resonance-stabilized x-ray free-electron laser oscillator for fundamental physics and precision metrology

    Science.gov (United States)

    Adams, B. W.; Kim, K.-J.

    2015-03-01

    An x-ray free-electron laser oscillator (XFELO) is a next-generation x-ray source, similar to free-electron laser oscillators at VUV and longer wavelengths but using crystals as high-reflectivity x-ray mirrors. Each output pulse from an XFELO is fully coherent with high spectral purity. The temporal coherence length can further be increased drastically, from picoseconds to microseconds or even longer, by phase-locking successive XFELO output pulses, using the narrow nuclear resonance lines of nuclei such as 57Fe as a reference. We show that the phase fluctuation due to the seismic activities is controllable and that due to spontaneous emission is small. The fluctuation of electron-bunch spacing contributes mainly to the envelope fluctuation but not to the phase fluctuation. By counting the number of standing-wave maxima formed by the output of the nuclear-resonance-stabilized (NRS) XFELO over an optically known length, the wavelength of the nuclear resonance can be accurately measured, possibly leading to a new length or frequency standard at x-ray wavelengths. A NRS-XFELO will be an ideal source for experimental x-ray quantum optics as well as other fundamental physics. The technique can be refined for other, narrower resonances such as 181Ta or 45Sc.

  15. X-ray comb generation from nuclear-resonance-stabilized x-ray free-electron laser oscillator for fundamental physics and precision metrology

    Directory of Open Access Journals (Sweden)

    B. W. Adams

    2015-03-01

    Full Text Available An x-ray free-electron laser oscillator (XFELO is a next-generation x-ray source, similar to free-electron laser oscillators at VUV and longer wavelengths but using crystals as high-reflectivity x-ray mirrors. Each output pulse from an XFELO is fully coherent with high spectral purity. The temporal coherence length can further be increased drastically, from picoseconds to microseconds or even longer, by phase-locking successive XFELO output pulses, using the narrow nuclear resonance lines of nuclei such as ^{57}Fe as a reference. We show that the phase fluctuation due to the seismic activities is controllable and that due to spontaneous emission is small. The fluctuation of electron-bunch spacing contributes mainly to the envelope fluctuation but not to the phase fluctuation. By counting the number of standing-wave maxima formed by the output of the nuclear-resonance-stabilized (NRS XFELO over an optically known length, the wavelength of the nuclear resonance can be accurately measured, possibly leading to a new length or frequency standard at x-ray wavelengths. A NRS-XFELO will be an ideal source for experimental x-ray quantum optics as well as other fundamental physics. The technique can be refined for other, narrower resonances such as ^{181}Ta or ^{45}Sc.

  16. X-Ray Comb Generation from Nuclear-Resonance-Stabilized X-Ray Free-Electron Laser Oscillator for Fundamental Physics and Precision Metrology

    Energy Technology Data Exchange (ETDEWEB)

    Adams, B. W.; Kim, K. -J.

    2015-03-31

    An x-ray free-electron laser oscillator (XFELO) is a next-generation x-ray source, similar to free-electron laser oscillators at VUV and longer wavelengths but using crystals as high-reflectivity x-ray mirrors. Each output pulse from an XFELO is fully coherent with high spectral purity. The temporal coherence length can further be increased drastically, from picoseconds to microseconds or even longer, by phase-locking successive XFELO output pulses, using the narrow nuclear resonance lines of nuclei such as Fe-57 as a reference. We show that the phase fluctuation due to the seismic activities is controllable and that due to spontaneous emission is small. The fluctuation of electron-bunch spacing contributes mainly to the envelope fluctuation but not to the phase fluctuation. By counting the number of standing-wave maxima formed by the output of the nuclear-resonance-stabilized (NRS) XFELO over an optically known length, the wavelength of the nuclear resonance can be accurately measured, possibly leading to a new length or frequency standard at x-ray wavelengths. A NRS-XFELO will be an ideal source for experimental x-ray quantum optics as well as other fundamental physics. The technique can be refined for other, narrower resonances such as Ta-181 or Sc-45.

  17. X-rays from magnetic intermediate mass Ap/Bp stars

    Science.gov (United States)

    Robrade, Jan

    2016-09-01

    The X-ray emission of magnetic intermediate mass Ap/Bp stars is reviewed and put into context of intrinsic as well as extrinsic hypotheses for its origin. New X-ray observations of Ap/Bp stars are presented and combined with an updated analysis of the available datasets, providing the largest sample of its type that is currently available. In the studied stars the X-ray detections are found predominantly among the more massive, hotter and more luminous targets. Their X-ray properties are quite diverse and beside strong soft X-ray emission significant magnetic activity is frequently present. While a connection between more powerful winds and brighter X-ray emission is expected in intrinsic models, the scatter in X-ray luminosity at given bolometric luminosity is so far unexplained and several observational features like X-ray light curves and flaring, luminosity distributions and spectral properties are often similar to those of low-mass stars. It remains to be seen if these features can be fully reproduced by magnetospheres of intermediate mass stars. The article discusses implications for magnetically confined wind-shock models (MCWS) and stellar magnetospheres under the assumption that the intrinsic model is applicable, but also examines the role of possible companions. Further, related magnetospheric phenomena are presented and an outlook on future perspectives is given.

  18. Magnetic moments in a gadolinium iron garnet studied by soft-X-ray magnetic circular dichroism

    NARCIS (Netherlands)

    Rudolf, P.; Sette, F.; Tjeng, L.H.; Meigs, G.; Chen, C.T.

    1992-01-01

    The magnetic moments of Gd and Fe in gadolinium iron garnet (Gd3Fe5O12) were probed at 77 and 300 K by soft-X-ray magnetic circular dichroism (SXMCD) measurements at the GdMa4,5 and at the FeL2,3 absorption edges. The SXMCD signal at each edge allows one to independently determine the magnetic order

  19. Visualization of magnetic dipolar interaction based on scanning transmission X-ray microscopy

    Science.gov (United States)

    Ohtori, Hiroyuki; Iwano, Kaoru; Mitsumata, Chiharu; Takeichi, Yasuo; Yano, Masao; Kato, Akira; Miyamoto, Noritaka; Shoji, Tetsuya; Manabe, Akira; Ono, Kanta

    2014-04-01

    Using scanning transmission X-ray microscopy (STXM), in this report we visualized the magnetic dipolar interactions in nanocrystalline Nd-Fe-B magnets and imaged their magnetization distributions at various applied fields. We calculated the magnetic dipolar interaction by analyzing the interaction between the magnetization at each point and those at the other points on the STXM image.

  20. Separated resonances in simultaneous capture and excitation of S/sup 15+/ in H/sub 2/ observed by K-x-ray--K-x-ray coincidences

    Energy Technology Data Exchange (ETDEWEB)

    Schulz, M.; Justiniano, E.; Schuch, R.; Mokler, P.H.; Reusch, S.

    1987-04-27

    We have measured cross sections for the correlated emission of two K x rays following the collision of hydrogenlike sulfur ions with H/sub 2/ in the energy range between 70 and 160 MeV. The observation of the two correlated x rays is interpreted as a resonant capture of a target electron accompanied by simultaneous excitation of the projectile in the collision (RTE). By our distinguishing between K..cap alpha.. and K..beta.. lines, contributions from KLL and KLn (ngreater than or equal toM) resonances could be determined independently.

  1. The influence of magnetic field geometry on magnetars X-ray spectra

    CERN Document Server

    Viganò, D; Zane, S; Turolla, R; Pons, J A; Miralles, J A

    2011-01-01

    Nowadays, the analysis of the X-ray spectra of magnetically powered neutron stars or magnetars is one of the most valuable tools to gain insight into the physical processes occurring in their interiors and magnetospheres. In particular, the magnetospheric plasma leaves a strong imprint on the observed X-ray spectrum by means of Compton up-scattering of the thermal radiation coming from the star surface. Motivated by the increased quality of the observational data, much theoretical work has been devoted to develop Monte Carlo (MC) codes that incorporate the effects of resonant Compton scattering in the modeling of radiative transfer of photons through the magnetosphere. The two key ingredients in this simulations are the kinetic plasma properties and the magnetic field (MF) configuration. The MF geometry is expected to be complex, but up to now only mathematically simple solutions (self-similar solutions) have been employed. In this work, we discuss the effects of new, more realistic, MF geometries on syntheti...

  2. Review - X-ray diffraction measurements in high magnetic fields and at high temperatures

    Directory of Open Access Journals (Sweden)

    Yoshifuru Mitsui, Keiichi Koyama and Kazuo Watanabe

    2009-01-01

    Full Text Available A system was developed measuring x-ray powder diffraction in high magnetic fields up to 5 T and at temperatures from 283 to 473 K. The stability of the temperature is within 1 K over 6 h. In order to examine the ability of the system, the high-field x-ray diffraction measurements were carried out for Si and a Ni-based ferromagnetic shape-memory alloy. The results show that the x-ray powder diffraction measurements in high magnetic fields and at high temperatures are useful for materials research.

  3. Resonant soft x-ray scattering and charge density waves in correlated systems

    NARCIS (Netherlands)

    Rusydi, Andrivo

    2006-01-01

    Summary This work describes results obtained on the study of charge density waves (CDW) in strongly correlated systems with a new experimental method: resonant soft x-ray scattering (RSXS). The basic motivation is the 1986 discovery by Bednorz and Müler of a new type of superconductor, based on Cu a

  4. 2p3d Resonant X-ray emission spectroscopy of cobalt compounds

    NARCIS (Netherlands)

    van Schooneveld, M.M.

    2013-01-01

    This manuscript demonstrates that 2p3d resonant X-ray emission spectroscopy (RXES) yields unique information on the chemically relevant valence electrons of transition metal atoms or ions. Experimental data on cobalt compounds and several theories were used hand-in-hand. In chapter 1 2p3d RXES was s

  5. Resonant soft x-ray scattering and charge density waves in correlated systems

    NARCIS (Netherlands)

    Rusydi, Andrivo

    2006-01-01

    Summary This work describes results obtained on the study of charge density waves (CDW) in strongly correlated systems with a new experimental method: resonant soft x-ray scattering (RSXS). The basic motivation is the 1986 discovery by Bednorz and Müler of a new type of superconductor, based on Cu

  6. Toroidal silicon polarization analyzer for resonant inelastic x-ray scattering.

    Science.gov (United States)

    Gao, Xuan; Casa, Diego; Kim, Jungho; Gog, Thomas; Li, Chengyang; Burns, Clement

    2016-08-01

    Resonant Inelastic X-ray Scattering (RIXS) is a powerful probe for studying electronic excitations in materials. Standard high energy RIXS measurements do not measure the polarization of the scattered x-rays, which is unfortunate since it carries information about the nature and symmetry of the excitations involved in the scattering process. Here we report the fabrication of thin Si-based polarization analyzers with a double-concave toroidal surface, useful for L-edge RIXS studies in heavier atoms such as the 5-d transition metals.

  7. Toroidal silicon polarization analyzer for resonant inelastic x-ray scattering

    Energy Technology Data Exchange (ETDEWEB)

    Gao, Xuan [Department of Physics, Western Michigan University, Kalamazoo, Michigan 49008-5252 (United States); Key Laboratory of Multi-scale Manufacturing Technology, Chongqing Institute of Green and Intelligent Technology, Chinese Academy of Sciences, Chongqing 400714 (China); Casa, Diego; Kim, Jungho; Gog, Thomas [Advanced Photon Source, Argonne National Laboratory, Argonne, Illinois 60439 (United States); Li, Chengyang [Department of Physics, Western Michigan University, Kalamazoo, Michigan 49008-5252 (United States); Department of Physics, South University of Science and Technology of China, Shenzhen 518055 (China); Burns, Clement [Department of Physics, Western Michigan University, Kalamazoo, Michigan 49008-5252 (United States)

    2016-08-15

    Resonant Inelastic X-ray Scattering (RIXS) is a powerful probe for studying electronic excitations in materials. Standard high energy RIXS measurements do not measure the polarization of the scattered x-rays, which is unfortunate since it carries information about the nature and symmetry of the excitations involved in the scattering process. Here we report the fabrication of thin Si-based polarization analyzers with a double-concave toroidal surface, useful for L-edge RIXS studies in heavier atoms such as the 5-d transition metals.

  8. Capability of Resonant Photoemission with Soft X-Rays in Rare-Earth Systems

    Science.gov (United States)

    Harasaki, Akiko; Tanaka, Arata; Jo, Takeo

    1993-07-01

    We theoretically discuss the capability of resonant photoemission with soft X-rays in clarifying the valence electronic state, by choosing Ce 4d core X-ray photoemission spectroscopy (4d XPS) at the Ce 3d threshold in CeRh3B2 with hexagonal crystal structure. On the basis of the Anderson model including multiplet splitting, we show that the dependence of 4d XPS on the energy and the linear polarization with respect to the hexagonal c-axis of the incident photon and the binding energy can be a powerful characteristic for probing a proposed uniaxial anisotropic distribution of 4f electrons.

  9. Strong higher-order resonant contributions to x-ray line polarization in hot plasmas

    CERN Document Server

    Shah, Chintan; Steinbrügge, Rene; Beilmann, Christian; Bernitt, Sven; Fritzsche, Stephan; Surzhykov, Andrey; López-Urrutia, José R Crespo; Tashenov, Stanislav

    2016-01-01

    We studied angular distributions of x rays emitted in resonant recombination of highly charged iron and krypton ions, resolving dielectronic, trielectronic, and quadruelectronic channels. A tunable electron beam drove these processes, inducing x rays registered by two detectors mounted along and perpendicular to the beam axis. The measured emission asymmetries comprehensively benchmarked full-order atomic calculations. We conclude that accurate polarization diagnostics of hot plasmas can only be obtained under the premise of inclusion of higher-order processes that were neglected in earlier work.

  10. X-ray topography analysis of acoustic wave fields in the SAW-resonator structures.

    Science.gov (United States)

    Roshchupkin, Dmitry V; Roshchupkina, Helen D; Irzhak, Dmitry V

    2005-11-01

    The formation of fields of standing surface acoustic waves (SAW) in LiNbO3 and La3Ga5SiO14 (LGS) crystals was studied by high-resolution topography method on a laboratory X-ray source. The fields of standing SAW were formed using SAW-resonator structures consisting of interdigital transducer (IDT) and reflecting gratings. The SAW amplitudes and power flow angles were measured by X-ray topography, diffraction in acoustic beam was visualized, and the SAW interaction with the crystal structure defects was studied.

  11. Building a Unified Computational Model for the Resonant X-Ray Scattering of Strongly Correlated Materials

    Energy Technology Data Exchange (ETDEWEB)

    Bansil, Arun [Northeastern Univ., Boston, MA (United States)

    2016-12-01

    Basic-Energy Sciences of the Department of Energy (BES/DOE) has made large investments in x-ray sources in the U.S. (NSLS-II, LCLS, NGLS, ALS, APS) as powerful enabling tools for opening up unprecedented new opportunities for exploring properties of matter at various length and time scales. The coming online of the pulsed photon source literally allows us to see and follow the dynamics of processes in materials at their natural timescales. There is an urgent need therefore to develop theoretical methodologies and computational models for understanding how x-rays interact with matter and the related spectroscopies of materials. The present project addressed aspects of this grand challenge of X-ray science. In particular, our Collaborative Research Team (CRT) focused on understanding and modeling of elastic and inelastic resonant X-ray scattering processes. We worked to unify the three different computational approaches currently used for modeling X-ray scattering—density functional theory, dynamical mean-field theory, and small-cluster exact diagonalization—to achieve a more realistic material-specific picture of the interaction between X-rays and complex matter. To achieve a convergence in the interpretation and to maximize complementary aspects of different theoretical methods, we concentrated on the cuprates, where most experiments have been performed. Our team included both US and international researchers, and it fostered new collaborations between researchers currently working with different approaches. In addition, we developed close relationships with experimental groups working in the area at various synchrotron facilities in the US. Our CRT thus helped toward enabling the US to assume a leadership role in the theoretical development of the field, and to create a global network and community of scholars dedicated to X-ray scattering research.

  12. Spin pumping through a topological insulator probed by x-ray detected ferromagnetic resonance

    Science.gov (United States)

    Figueroa, A. I.; Baker, A. A.; Collins-McIntyre, L. J.; Hesjedal, T.; van der Laan, G.

    2016-02-01

    In the field of spintronics, the generation of a pure spin current (without macroscopic charge flow) through spin pumping of a ferromagnetic (FM) layer opens up the perspective of a new generation of dissipation-less devices. Microwave driven ferromagnetic resonance (FMR) can generate a pure spin current that enters adjacent layers, allowing for both magnetization reversal (through spin-transfer torque) and to probe spin coherence in non-magnetic materials. However, standard FMR is unable to probe multilayer dynamics directly, since the measurement averages over the contributions from the whole system. The synchrotron radiation-based technique of x-ray detected FMR (XFMR) offers an elegant solution to this drawback, giving access to element-, site-, and layer-specific dynamical measurements in heterostructures. In this work, we show how XFMR has provided unique information to understand spin pumping and spin transfer torque effects through a topological insulator (TI) layer in a pseudo-spin valve heterostructure. We demonstrate that TIs function as efficient spin sinks, while also allowing a limited dynamic coupling between ferromagnetic layers. These results shed new light on the spin dynamics of this novel class of materials, and suggest future directions for the development of room temperature TI-based spintronics.

  13. Investigation of self-filtering unstable resonator for soft x-ray lasers

    Science.gov (United States)

    Ghani-Moghadam, G.; Farahbod, A. H.

    2016-07-01

    In this paper, it is proposed that the self-filtering unstable resonator (SFUR) is suitable for soft x-ray lasers which have active medium with a short-gain-lifetime. In order to evaluate the idea, we have analyzed the self-filtering unstable resonator in two dimensions with Ne-like Fe soft x-ray active medium for transitions 2p5 3 p → 2p5 3 s and 3d9 4 d → 3d9 4 p at 25.5 nm. The role of field-limiting aperture in mode propagation has been shown. Moreover, beam quality factor M2 has been calculated and output mode behavior studied and compared with a plane-parallel (PP) resonator of equal length. The calculations indicate that the M2 factor in SFUR resonator is smaller than PP resonator and therefore output beam divergence is lower and the mode quality is much better. It is expected that a high quality beam of soft x-ray laser with brightness of the order 1013 W / cm2 sr and energy more than 10 nJ may be achievable with a properly designed diffraction-filtered unstable resonator.

  14. Role of screening and angular distributions in resonant soft-x-ray emission of CO

    Energy Technology Data Exchange (ETDEWEB)

    Skytt, P.; Glans, P.; Gunnelin, K. [Uppsala Univ. (Sweden)] [and others

    1997-04-01

    In the present work the authors focus on two particular properties of resonant X-ray emission, namely core hole screening of the excited electron, and anisotropy caused by the polarization of the exciting synchrotron radiation. The screening of the core hole by the excited electron causes energy shifts and intensity variations in resonant spectra compared to the non-resonant case. The linear polarization of the synchrotron radiation and the dipole nature of the absorption process create a preferential alignment selection of the randomly oriented molecules in the case of resonant excitation, producing an anisotropy in the angular distribution of the emitted X-rays. The authors have chosen CO for this study because this molecule has previously served as a showcase for non-resonant X-ray emission, mapping the valence electronic structure differently according to the local selection rules. With the present work they take interest in how this characteristic feature of the spectroscopy is represented in the resonant case.

  15. Double-confocal resonator for X-ray generation via intracavity Thomson scattering

    Energy Technology Data Exchange (ETDEWEB)

    Xie, M. [Lawrence Berkeley Lab., CA (United States)

    1995-12-31

    There has been a growing interest in developing compact X-ray sources through Thomson scattering of a laser beam by a relativistic electron beam. For higher X-ray flux it is desirable to have the scattering to occur inside an optical resonator where the laser power is higher. In this paper I propose a double-confocal resonator design optimized for head-on Thomson scattering inside an FEL oscillator and analyze its performance taking into account the diffraction and FEL gain. A double confocal resonator is equivalent to two confocal resonators in series. Such a resonator has several advantages: it couples electron beam through and X-ray out of the cavity with holes on cavity mirrors, thus allowing the system to be compact; it supports the FEL mode with minimal diffraction loss through the holes; it provides a laser focus in the forward direction for a better mode overlap with the electron beam; and it provides a focus at the same location in the backward direction for higher Thomson scattering efficiency; in addition, the mode size at the focal point and hence the Rayleigh range can be adjusted simply through intracavity apertures; furthermore, it gives a large mode size at the mirrors to reduce power loading. Simulations as well as analytical results will be presented. Also other configurations of intracavity Thomson scattering where the double-confocal resonator could be useful will be discussed.

  16. Prospects for x-ray polarimetry measurements of magnetic fields in magnetized liner inertial fusion plasmas

    Energy Technology Data Exchange (ETDEWEB)

    Lynn, Alan G., E-mail: lynn@ece.unm.edu; Gilmore, Mark [Department of Electrical and Computer Engineering, University of New Mexico, Albuquerque, New Mexico 87131 (United States)

    2014-11-15

    Magnetized Liner Inertial Fusion (MagLIF) experiments, where a metal liner is imploded to compress a magnetized seed plasma may generate peak magnetic fields ∼10{sup 4} T (100 Megagauss) over small volumes (∼10{sup −10}m{sup 3}) at high plasma densities (∼10{sup 28}m{sup −3}) on 100 ns time scales. Such conditions are extremely challenging to diagnose. We discuss the possibility of, and issues involved in, using polarimetry techniques at x-ray wavelengths to measure magnetic fields under these extreme conditions.

  17. Prospects for x-ray polarimetry measurements of magnetic fields in magnetized liner inertial fusion plasmas

    Science.gov (United States)

    Lynn, Alan G.; Gilmore, Mark

    2014-11-01

    Magnetized Liner Inertial Fusion (MagLIF) experiments, where a metal liner is imploded to compress a magnetized seed plasma may generate peak magnetic fields ˜104 T (100 Megagauss) over small volumes (˜10-10m3) at high plasma densities (˜1028m-3) on 100 ns time scales. Such conditions are extremely challenging to diagnose. We discuss the possibility of, and issues involved in, using polarimetry techniques at x-ray wavelengths to measure magnetic fields under these extreme conditions.

  18. Prospects for x-ray polarimetry measurements of magnetic fields in magnetized liner inertial fusion plasmas.

    Science.gov (United States)

    Lynn, Alan G; Gilmore, Mark

    2014-11-01

    Magnetized Liner Inertial Fusion (MagLIF) experiments, where a metal liner is imploded to compress a magnetized seed plasma may generate peak magnetic fields ∼10(4) T (100 Megagauss) over small volumes (∼10(-10)m(3)) at high plasma densities (∼10(28)m(-3)) on 100 ns time scales. Such conditions are extremely challenging to diagnose. We discuss the possibility of, and issues involved in, using polarimetry techniques at x-ray wavelengths to measure magnetic fields under these extreme conditions.

  19. A cooled avalanche photodiode detector for X-ray magnetic diffraction experiments

    CERN Document Server

    Kishimoto, S; Ito, M

    2001-01-01

    A cooled avalanche photodiode (APD) detector was developed for X-ray magnetic diffraction experiments. A stack of four silicon APDs was cooled down to 243 K by a thermoelectric cooler. The energy widths of 0.89 and 1.55 keV (FWHM) were obtained for 8.05 keV X-rays at 1x10 sup 6 s sup - sup 1 and for 16.53 keV X-rays at 2x10 sup 6 s sup - sup 1 , respectively. Test measurements of X-ray magnetic diffraction were executed using a terbium single crystal and white synchrotron radiation. A peak width of (1 0 3) reflection (5.4 keV) was roughly three times wider than that with a high-purity germanium detector.

  20. A multiplexed high-resolution imaging spectrometer for resonant inelastic soft X-ray scattering spectroscopy.

    Science.gov (United States)

    Warwick, Tony; Chuang, Yi De; Voronov, Dmitriy L; Padmore, Howard A

    2014-07-01

    The optical design of a two-dimensional imaging soft X-ray spectrometer is described. A monochromator will produce a dispersed spectrum in a narrow vertical illuminated stripe (∼2 µm wide by ∼2 mm tall) on a sample. The spectrometer will use inelastically scattered X-rays to image the extended field on the sample in the incident photon energy direction (vertical), resolving the incident photon energy. At the same time it will image and disperse the scattered photons in the orthogonal (horizontal) direction, resolving the scattered photon energy. The principal challenge is to design a system that images from the flat-field illumination of the sample to the flat field of the detector and to achieve sufficiently high spectral resolution. This spectrometer provides a completely parallel resonant inelastic X-ray scattering measurement at high spectral resolution (∼30,000) over the energy bandwidth (∼5 eV) of a soft X-ray absorption resonance.

  1. 4 f excitations in Ce Kondo lattices studied by resonant inelastic x-ray scattering

    Science.gov (United States)

    Amorese, A.; Dellea, G.; Fanciulli, M.; Seiro, S.; Geibel, C.; Krellner, C.; Makarova, I. P.; Braicovich, L.; Ghiringhelli, G.; Vyalikh, D. V.; Brookes, N. B.; Kummer, K.

    2016-04-01

    The potential of resonant inelastic soft x-ray scattering to measure 4 f crystal electric-field excitation spectra in Ce Kondo lattices has been examined. Spectra have been obtained for several Ce systems and show a well-defined structure determined by crystal-field, spin-orbit, and charge-transfer excitations only. The spectral shapes of the excitation spectra can be well understood in the framework of atomic multiplet calculations. For CeCu2Si2 we found notable disagreement between the inelastic x-ray-scattering spectra and theoretical calculations when using the crystal-field scheme proposed from inelastic neutron scattering. Modified sets of crystal-field parameters yield better agreement. Our results also show that, with the very recent improvements of soft x-ray spectrometers in resolution to below 30 meV at the Ce M4 ,5 edges, resonant inelastic x-ray scattering could be an ideal tool to determine the crystal-field scheme in Ce Kondo lattices and other rare-earth compounds.

  2. Magnetic fields, winds and X-rays of massive stars in the Orion Nebula Cluster

    CERN Document Server

    Petit, V; Drissen, L; Montmerle, T; Alecian, E

    2008-01-01

    In massive stars, magnetic fields are thought to confine the outflowing radiatively-driven wind, resulting in X-ray emission that is harder, more variable and more efficient than that produced by instability-generated shocks in non-magnetic winds. Although magnetic confinement of stellar winds has been shown to strongly modify the mass-loss and X-ray characteristics of massive OB stars, we lack a detailed understanding of the complex processes responsible. The aim of this study is to examine the relationship between magnetism, stellar winds and X-ray emission of OB stars. In conjunction with a Chandra survey of the Orion Nebula Cluster, we carried out spectropolarimatric ESPaDOnS observations to determine the magnetic properties of massive OB stars of this cluster.

  3. Effects of dispersion and absorption in resonant Bragg diffraction of x-rays.

    Science.gov (United States)

    Lovesey, S W; Scagnoli, V; Dobrynin, A N; Joly, Y; Collins, S P

    2014-03-26

    Resonant diffraction of x-rays by crystals with anisotropic optical properties is investigated theoretically, to assess how the intensity of a Bragg spot is influenced by effects related to dispersion (birefringence) and absorption (dichroism). Starting from an exact but opaque expression, simple analytic results are found to expose how intensity depends on dispersion and absorption in the primary and secondary beams and, also, the azimuthal angle (rotation of the crystal about the Bragg wavevector). If not the full story for a given application, our results are more than adequate to explore consequences of dispersion and absorption in the intensity of a Bragg spot. Results are evaluated for antiferromagnetic copper oxide, and low quartz. For CuO, one of our results reproduces all salient features of a previously published simulation of the azimuthal-angle dependence of a magnetic Bragg peak. It is transparent in our analytic result that dispersion and absorption effects alone cannot reproduce published experimental data. Available data for the azimuthal-angle dependence of space-group forbidden reflections (0,0, l), with l ≠ 3n, of low quartz depart from symmetry imposed by the triad axis of rotation symmetry. The observed asymmetry can be induced by dispersion and absorption even though absorption coefficients are constant, independent of the azimuthal angle, in this class of reflections.

  4. Soft-X-ray magnetic circular dichroism : a new technique for probing magnetic properties of magnetic surfaces and ultrathin films

    NARCIS (Netherlands)

    Tjeng, L.H.; Idzerda, Y.U.; Rudolf, P.; Sette, F.; Chen, C.T.

    1992-01-01

    We demonstrate the feasibility of applying the novel soft-X-ray magnetic circular dichroism (SXMCD) technique to investigate the magnetic properties of magnetic surfaces and uitrathin films. Measurements have been carried out on Ni films of various thickness on a Cu(100) substrate at the Ni L2,3 abs

  5. Calibration standard of body tissue with magnetic nanocomposites for MRI and X-ray imaging

    Science.gov (United States)

    Rahn, Helene; Woodward, Robert; House, Michael; Engineer, Diana; Feindel, Kirk; Dutz, Silvio; Odenbach, Stefan; StPierre, Tim

    2016-05-01

    We present a first study of a long-term phantom for Magnetic Resonance Imaging (MRI) and X-ray imaging of biological tissues with magnetic nanocomposites (MNC) suitable for 3-dimensional and quantitative imaging of tissues after, e.g. magnetically assisted cancer treatments. We performed a cross-calibration of X-ray microcomputed tomography (XμCT) and MRI with a joint calibration standard for both imaging techniques. For this, we have designed a phantom for MRI and X-ray computed tomography which represents biological tissue enriched with MNC. The developed phantoms consist of an elastomer with different concentrations of multi-core MNC. The matrix material is a synthetic thermoplastic gel, PermaGel (PG). The developed phantoms have been analyzed with Nuclear Magnetic Resonance (NMR) Relaxometry (Bruker minispec mq 60) at 1.4 T to obtain R2 transverse relaxation rates, with SQUID (Superconducting QUantum Interference Device) magnetometry and Inductively Coupled Plasma Mass Spectrometry (ICP-MS) to verify the magnetite concentration, and with XμCT and 9.4 T MRI to visualize the phantoms 3-dimensionally and also to obtain T2 relaxation times. A specification of a sensitivity range is determined for standard imaging techniques X-ray computed tomography (XCT) and MRI as well as with NMR. These novel phantoms show a long-term stability over several months up to years. It was possible to suspend a particular MNC within the PG reaching a concentration range from 0 mg/ml to 6.914 mg/ml. The R2 relaxation rates from 1.4 T NMR-relaxometry show a clear connection (R2=0.994) with MNC concentrations between 0 mg/ml and 4.5 mg/ml. The MRI experiments have shown a linear correlation of R2 relaxation and MNC concentrations as well but in a range between MNC concentrations of 0 mg/ml and 1.435 mg/ml. It could be shown that XμCT displays best moderate and high MNC concentrations. The sensitivity range for this particular XμCT apparatus yields from 0.569 mg/ml to 6.914 mg/ml. The

  6. Improving the spatial resolution of a soft X-ray Charge Coupled Device used for Resonant Inelastic X-ray Scattering

    Science.gov (United States)

    Soman, M. R.; Hall, D. J.; Tutt, J. H.; Murray, N. J.; Holland, A. D.; Schmitt, T.; Raabe, J.; Schmitt, B.

    2011-11-01

    The Super Advanced X-ray Emission Spectrometer (SAXES) at the Advanced Resonant Scattering (ADRESS) beamline of the Swiss Light Source is a high-resolution X-ray spectrometer used as an end station for Resonant Inelastic X-ray Scattering from 400 eV to 1600 eV. Through the dispersion of photons across a CCD, the energy of scattered photons may be determined by their detected spatial position. The limiting factor of the energy resolution is currently the spatial resolution achieved with the CCD, reported at 24 μm FWHM. For this energy range the electron clouds are formed by interactions in the `field free' region of the back-illuminated CCD. These clouds diffuse in all directions whilst being attracted to the electrodes, leading to events that are made up of signals in multiple pixels. The spreading of the charge allows centroiding techniques to be used to improve the CCD spatial resolution and therefore improve the energy resolution of SAXES. The PolLux microscopy beamline at the SLS produces an X-ray beam with a diameter of 20 nm. The images produced from scanning the narrow beam across CCD pixels (13.5 × 13.5 μm2) can aid in the production of event recognition algorithms, allowing the matching of event profiles to photon interactions in a specific region of a pixel. Through the use of this information software analysis can be refined with the aim of improving the energy resolution.

  7. A von Hamos x-ray spectrometer based on a segmented-type diffraction crystal for single-shot x-ray emission spectroscopy and time-resolved resonant inelastic x-ray scattering studies.

    Science.gov (United States)

    Szlachetko, J; Nachtegaal, M; de Boni, E; Willimann, M; Safonova, O; Sa, J; Smolentsev, G; Szlachetko, M; van Bokhoven, J A; Dousse, J-Cl; Hoszowska, J; Kayser, Y; Jagodzinski, P; Bergamaschi, A; Schmitt, B; David, C; Lücke, A

    2012-10-01

    We report on the design and performance of a wavelength-dispersive type spectrometer based on the von Hamos geometry. The spectrometer is equipped with a segmented-type crystal for x-ray diffraction and provides an energy resolution in the order of 0.25 eV and 1 eV over an energy range of 8000 eV-9600 eV. The use of a segmented crystal results in a simple and straightforward crystal preparation that allows to preserve the spectrometer resolution and spectrometer efficiency. Application of the spectrometer for time-resolved resonant inelastic x-ray scattering and single-shot x-ray emission spectroscopy is demonstrated.

  8. Photoinduced molecular chirality probed by ultrafast resonant X-ray spectroscopy

    Directory of Open Access Journals (Sweden)

    Jérémy R. Rouxel

    2017-07-01

    Full Text Available Recently developed circularly polarized X-ray light sources can probe the ultrafast chiral electronic and nuclear dynamics through spatially localized resonant core transitions. We present simulations of time-resolved circular dichroism signals given by the difference of left and right circularly polarized X-ray probe transmission following an excitation by a circularly polarized optical pump with the variable time delay. Application is made to formamide which is achiral in the ground state and assumes two chiral geometries upon optical excitation to the first valence excited state. Probes resonant with various K-edges (C, N, and O provide different local windows onto the parity breaking geometry change thus revealing the enantiomer asymmetry.

  9. 25 Tesla pulsed-high-magnetic-field system for soft X-ray spectroscopy

    Energy Technology Data Exchange (ETDEWEB)

    Hayashi, M., E-mail: mhaya@imr.tohoku.ac.jp [Institute for Materials Research, Tohoku University, Sendai 980-8577 (Japan); Narumi, Y.; Nojiri, H. [Institute for Materials Research, Tohoku University, Sendai 980-8577 (Japan); Nakamura, T.; Hirono, T.; Kinoshita, T. [JASRI/SPring-8, Sayo, Hyogo 679-5198 (Japan); Kodama, K. [Department of Mechanical Engineering, Nara National College of Technology, Nara 639-1080 (Japan); Kindo, K. [Institute for Solid State Physics, University of Tokyo, Kashiwa 277-8581 (Japan)

    2011-04-15

    Research highlights: {yields} We have developed a 25 T pulsed magnetic field system for soft X-ray MCD. {yields} The new capacitor bank can generate a field in the bipolar mode. {yields} We measured the Soft X-ray MCD of paramagnetic Gd{sub 2}O{sub 3} up to 25 T. - Abstract: We have developed a 25 T pulsed high magnetic field system for soft X-ray Magnetic Circular Dichroism: XMCD. The ultra-high vacuum chamber with a pulse magnet coil is installed. By using a newly developed bipolar capacitor bank, the XMCD of paramagnetic Gd{sub 2}O{sub 3} at the M{sub 5} and the M{sub 4} edges was clearly observed at low temperatures. The present system is capable of measuring XMCD of field induced moments in various compounds including paramagnets and antiferromagnets.

  10. Thermal X-ray emission from massive, fast rotating, highly magnetized white dwarfs

    CERN Document Server

    Caceres, D L; Coelho, J G; de Lima, R C R; Rueda, Jorge A

    2016-01-01

    There is solid observational evidence on the existence of massive, $M\\sim 1~M_\\odot$, highly magnetized white dwarfs (WDs) with surface magnetic fields up to $B\\sim 10^9$ G. We show that, if in addition to these features, the star is fast rotating, it can become a rotation-powered pulsar-like WD and emit detectable high-energy radiation. We infer the values of the structure parameters (mass, radius, moment of inertia), magnetic field, rotation period and spin-down rates of a WD pulsar death-line. We show that WDs above the death-line emit blackbody radiation in the soft X-ray band via the magnetic polar cap heating by back flowing pair-created particle bombardment and discuss as an example the X-ray emission of soft gamma-repeaters and anomalous X-ray pulsars within the WD model.

  11. Hard X-Ray Burst Detected From Caltech Plasma Jet Experiment Magnetic Reconnection Event

    Science.gov (United States)

    Marshall, Ryan S.; Bellan, Paul M.

    2016-10-01

    In the Caltech plasma jet experiment a 100 kA MHD driven jet becomes kink unstable leading to a Rayleigh-Taylor instability that quickly causes a magnetic reconnection event. Movies show that the Rayleigh-Taylor instability is simultaneous with voltage spikes across the electrodes that provide the current that drives the jet. Hard x-rays between 4 keV and 9 keV have now been observed using an x-ray scintillator detector mounted just outside of a kapton window on the vacuum chamber. Preliminary results indicate that the timing of the x-ray burst coincides with a voltage spike on the electrodes occurring in association with the Rayleigh-Taylor event. The x-ray signal accompanies the voltage spike and Rayleigh-Taylor event in approximately 50% of the shots. A possible explanation for why the x-ray signal is sometimes missing is that the magnetic reconnection event may be localized to a specific region of the plasma outside the line of sight of the scintillator. The x-ray signal has also been seen accompanying the voltage spike when no Rayleigh-Taylor is observed. This may be due to the interframe timing on the camera being longer than the very short duration of the Rayleigh-Taylor instability.

  12. Identification of inversion domains in KTiOPO{sub 4}via resonant X-ray diffraction

    Energy Technology Data Exchange (ETDEWEB)

    Fabrizi, Federica, E-mail: federica.fabrizi@diamond.ac.uk [Diamond Light Source, Harwell Science and Innovation Campus, Didcot, OX11 0DE (United Kingdom); Thomas, Pamela A. [Department of Physics, University of Warwick, Coventry, CV4 7AL (United Kingdom); Nisbet, Gareth; Collins, Stephen P. [Diamond Light Source, Harwell Science and Innovation Campus, Didcot, OX11 0DE (United Kingdom)

    2015-05-14

    The identification and high-resolution mapping of the absolute crystallographic structure in multi-domain ferroelectric KTiOPO{sub 4} is achieved through a novel synchrotron X-ray diffraction method. On a single Bragg reflection, the intensity ratio in resonant diffraction below and above the Ti absorption K edge demonstrates a domain contrast up to a factor of ∼270, thus implementing a non-contact, non-destructive imaging technique with micrometre spatial resolution, applicable to samples of arbitrarily large dimensions. A novel method is presented for the identification of the absolute crystallographic structure in multi-domain polar materials such as ferroelectric KTiOPO{sub 4}. Resonant (or ‘anomalous’) X-ray diffraction spectra collected across the absorption K edge of Ti (4.966 keV) on a single Bragg reflection demonstrate a huge intensity ratio above and below the edge, providing a polar domain contrast of ∼270. This allows one to map the spatial domain distribution in a periodically inverted sample, with a resolution of ∼1 µm achieved with a microfocused beam. This non-contact, non-destructive technique is well suited for samples of large dimensions (in contrast with traditional resonant X-ray methods based on diffraction from Friedel pairs), and its potential is particularly relevant in the context of physical phenomena connected with an absence of inversion symmetry, which require characterization of the underlying absolute atomic structure (such as in the case of magnetoelectric coupling and multiferroics)

  13. A Novel X-ray Diffractometer for the Florida Split Coil 25 Tesla Magnet

    Science.gov (United States)

    Wang, Shengyu; Kovalev, Alexey; Suslov, Alexey; Siegrist, Theo

    2014-03-01

    At National High Magnetic Field Laboratory (NHMFL), we are developing a unique X-ray diffractometer for the 25 Tesla Florida Split Coil Magnet for scattering experiments under extremely high static magnetic fields. The X-ray source is a sealed tube (copper or molybdenum anode), connected to the magnet by an evacuated beam tunnel. The detectors are either an image plate or a silicon drift detector, with the data acquisition system based on LabVIEW. Our preliminary experimental results showed that the performance of the detector electronics and the X-ray generator is reliable in the fringe magnetic fields produced at the highest field of 25 T. Using this diffractometer, we will make measurements on standard samples, such as LaB6, Al2O3 and Si, to calibrate the diffraction system. Magnetic samples, such as single crystal HoMnO3 and stainless steel 301 alloys will be measured subsequently. The addition of X-ray diffraction to the unique split coil magnet will significantly expand the NHMFL experimental capabilities. Therefore, external users will be able to probe spin - lattice interactions at static magnetic fields up to 25T. This project is supported by NSF-DMR Award No.1257649. NHMFL is supported by NSF Cooperative Agreement No. DMR-1157490, the State of Florida, and the U.S. DoE.

  14. X-ray analysis of oxygen-induced perpendicular magnetic anisotropy in Pt/Co/AlO{sub x} trilayers

    Energy Technology Data Exchange (ETDEWEB)

    Manchon, A. [SPINTEC, URA 2512 CEA/CNRS, CEA/Grenoble, 38054 Grenoble Cedex 9 (France)], E-mail: aurelien.manchon@m4x.org; Pizzini, S.; Vogel, J.; Uhlir, V. [Institut Neel, CNRS/UJF, B.P. 166, 38042 Grenoble Cedex 9 (France); Lombard, L.; Ducruet, C.; Auffret, S.; Rodmacq, B.; Dieny, B. [SPINTEC, URA 2512 CEA/CNRS, CEA/Grenoble, 38054 Grenoble Cedex 9 (France); Hochstrasser, M. [Laboratory for Solid State Physics, ETH Zuerich, 8093 Zuerich (Switzerland); Panaccione, G. [Laboratory TASC, INFM-CNR, Area Science Park, S.S.14, Km 163.5, I-34012, Trieste (Italy)

    2008-07-15

    X-ray spectroscopy measurements have been performed on a series of Pt/Co/AlO{sub x} trilayers to investigate the role of Co oxidation in the perpendicular magnetic anisotropy of the Co/AlO{sub x} interface. It is observed that high temperature annealing modifies the magnetic properties of the Co layer, inducing an enhancement of the perpendicular magnetic anisotropy. The microscopic structural properties are analyzed via X-ray Absorption Spectroscopy, X-ray Magnetic Circular Dichroism and X-ray Photoelectron Spectroscopy measurements. It is shown that annealing enhances the amount of interfacial oxide, which may be at the origin of a strong perpendicular magnetic anisotropy.

  15. Monochromatic X-ray propagation in multi-Z media for imaging and diagnostics including Kα Resonance Fluorescence

    Science.gov (United States)

    Westphal, Maximillian; Lim, Sara; Nahar, Sultana; Pradhan, Anil

    2016-05-01

    Aimed at monochromatic X-ray imaging and therapy, broadband, monochromatic, and quasi-monochromatic X-ray sources and propagation through low and high-Z (HZ) media were studied with numerically and experimentally. Monte Carlo simulations were performed using the software package Geant4, and a new code Photx, to simulate X-ray image contrast, depth of penetration, and total attenuation. The data show that monochromatic and quasi-monochromatic X-rays achieve improved contrast at lower absorbed radiation doses compared to conventional broadband 120 kV or CT scans. Experimental quasi-monochromatic high-intensity laser-produced plasma sources and monochromatic synchrotron beam data are compared. Physical processes responsible for X-ray photoexcitation and absorption are numerically modelled, including a novel mechanism for accelerating Kα resonance fluorescence via twin monochromatic X-ray beam. Potential applications are medical diagnostics and high-Z material detection. Acknowledgement: Ohio Supercomputer Center, Columbus, OH.

  16. X-ray Pulsars

    CERN Document Server

    Walter, Roland

    2016-01-01

    X-ray pulsars shine thanks to the conversion of the gravitational energy of accreted material to X-ray radiation. The accretion rate is modulated by geometrical and hydrodynamical effects in the stellar wind of the pulsar companions and/or by instabilities in accretion discs. Wind driven flows are highly unstable close to neutron stars and responsible for X-ray variability by factors $10^3$ on time scale of hours. Disk driven flows feature slower state transitions and quasi periodic oscillations related to orbital motion and precession or resonance. On shorter time scales, and closer to the surface of the neutron star, X-ray variability is dominated by the interactions of the accreting flow with the spinning magnetosphere. When the pulsar magnetic field is large, the flow is confined in a relatively narrow accretion column, whose geometrical properties drive the observed X-ray emission. In low magnetized systems, an increasing accretion rate allows the ignition of powerful explosive thermonuclear burning at t...

  17. X-ray resonant scattering study of the quadrupolar order in UPd3

    DEFF Research Database (Denmark)

    McMorrow, D.F.; McEwen, K.A.; Steigenberger, U.

    2001-01-01

    Quadrupolar ordering in a 5f electron system has been observed directly for the first time, using x-ray scattering techniques. In UPd(3) at low temperatures satellite peaks appear at (1, 0, l) (orthorhombic notation) with I odd and even. Both sets of peaks show a resonant enhancement...... of the scattering at the M(IV) edge of U. At resonance, the dominant scattering of the 1 odd peaks occurs in the unrotated polarization channel, whereas for I even a significant rotated component is found. These results are discussed in terms of possible structures of the antiferroquadrupolar phases....

  18. Period Clustering of the Anomalous X-Ray Pulsars and Magnetic Field Decay in Magnetars.

    Science.gov (United States)

    Colpi; Geppert; Page

    2000-01-20

    We confront theoretical models for the rotational, magnetic, and thermal evolution of an ultramagnetized neutron star, or magnetar, with available data on the anomalous X-ray pulsars (AXPs). We argue that, if the AXPs are interpreted as magnetars, their clustering of spin periods between 6 and 12 s (observed at present in this class of objects), their period derivatives, their thermal X-ray luminosities, and the association of two of them with young supernova remnants can only be understood globally if the magnetic field in magnetars decays significantly on a timescale of the order of 104 yr.

  19. Investigation of electronic order using resonant soft X-ray diffraction

    Energy Technology Data Exchange (ETDEWEB)

    Schlappa, J.

    2006-12-01

    The aim of this PhD work was the application of resonant soft X-ray diffraction technique for the investigation of electronic order in transition metal oxides at the TM L{sub 2,3}-edge, trying to obtain a quantitative understanding of the data. The method was first systematically explored through application to a model system in order to test the feasibility of the technique and to understand of how X-ray optical effects have to be taken into account. Two more complex systems were investigated; stripe order in La{sub 1.8}Sr{sub 0.2}NiO{sub 4} and charge and orbital order in Fe{sub 3}O{sub 4}. The main focus of the work was on the spectroscopic potential of the technique, trying to obtain a level of quantitative description of the data. For X-ray absorption spectroscopy (XAS) from transition metal oxides, cluster configuration interaction calculation provides a powerful and realistic microscopic theory. In the frame work of this thesis cluster theory, considering explicit hybridization effects between the TM-ion and the surrounding oxygen ligands, has been applied for the first time to describe resonant diffraction data. (orig.)

  20. Resonant x-ray emission from gas-phase TiCl{sub 4}

    Energy Technology Data Exchange (ETDEWEB)

    Hague, C.F.; Tronc, M. [Universite Pierre et Marie Curie, Paris (France); De Groot, F. [Univ. of Groningen (Netherlands)] [and others

    1997-04-01

    Resonant x-ray emission spectroscopy (RXES) has proved to be a powerful tool for studying the electronic structure of condensed matter. Over the past few years it has been used mainly for studying the valence bands of solids and condensed molecules. Very recently the advent of high brightness photon beams provided by third generation synchrotron radiation source undulators, associated with efficient x-ray emission spectrometers has made it possible to perform experiments on free diatomic molecular systems. RXE spectra of free molecules are of prime importance to gain insight into their electronic structure and bonding as they reflect the symmetry of orbitals engaged in the two-electron, two-step process with the l = 0, {+-}2 parity-conserving selection rule, and are free from solid state effects which can introduce difficulties in the interpretation. They provide information (more so than XAS) on the core excited states, and, when performed at fixed incident photon energy as a function of the emitted photon energy, on the electronic excitation (charge transfer, multiplet states). Moreover the anisotropy of the angular distribution of resonant x-ray emission affects the relative intensity of the emission peaks and provides information concerning the symmetries of final states. This is a preliminary report on what are the first RXE spectra of a 3d transition metal complex in the gas phase. The experiment concerns the Ti 3d {yields}2p emission spectrum of TiCl{sub 4} over the 450 to 470 eV region.

  1. Direct experimental determination of spiral spin structures via the dichroism extinction effect in resonant elastic soft x-ray scattering

    Science.gov (United States)

    Zhang, S. L.; van der Laan, G.; Hesjedal, T.

    2017-09-01

    Long-wavelength spin spiral structures are ubiquitous in a large variety of magnetic materials. The detailed magnetic structure can take many variations owing to their different physical origins. Therefore, the unambiguous structural determination is crucial for understanding these spin systems, though such a task is experimentally challenging. Here, we show that ordered spin spiral structures can be fully determined in a single measurement by dichroic resonant elastic x-ray scattering using circularly polarized light. It is found that at certain geometrical conditions, the circular dichroism of the diffraction vanishes completely, revealing a one-to-one correspondence with the spin structure. We demonstrate both theoretically and experimentally this experimental principle, which allows for unambiguous structure determination immediately from the measured signal, whereby no modeling-based data refinement is needed. This largely expands the capabilities of conventional magnetic characterization techniques.

  2. Selective gating to vibrational modes through resonant X-ray scattering

    Science.gov (United States)

    Couto, Rafael C.; Cruz, Vinícius V.; Ertan, Emelie; Eckert, Sebastian; Fondell, Mattis; Dantz, Marcus; Kennedy, Brian; Schmitt, Thorsten; Pietzsch, Annette; Guimarães, Freddy F.; Ågren, Hans; Gel'Mukhanov, Faris; Odelius, Michael; Kimberg, Victor; Föhlisch, Alexander

    2017-01-01

    The dynamics of fragmentation and vibration of molecular systems with a large number of coupled degrees of freedom are key aspects for understanding chemical reactivity and properties. Here we present a resonant inelastic X-ray scattering (RIXS) study to show how it is possible to break down such a complex multidimensional problem into elementary components. Local multimode nuclear wave packets created by X-ray excitation to different core-excited potential energy surfaces (PESs) will act as spatial gates to selectively probe the particular ground-state vibrational modes and, hence, the PES along these modes. We demonstrate this principle by combining ultra-high resolution RIXS measurements for gas-phase water with state-of-the-art simulations.

  3. Determination of the absolute chirality of tellurium using resonant diffraction with circularly polarized x-rays.

    Science.gov (United States)

    Tanaka, Y; Collins, S P; Lovesey, S W; Matsumami, M; Moriwaki, T; Shin, S

    2010-03-31

    Many proteins, sugars and pharmaceuticals crystallize into two forms that are mirror images of each other (enantiomers) like our right and left hands. Tellurium is one enantiomer having a space group pair, P3(1)21 (right-handed screw) and P3(2)21 (left-handed screw). X-ray diffraction with dispersion correction terms has been playing an important role in determining the handedness of enantiomers for a long time. However, this approach is not applicable for an elemental crystal such as tellurium or selenium. We have demonstrated that positive and negative circularly polarized x-rays at the resonant energy of tellurium can be used to absolutely distinguish right from left tellurium. This method is applicable to chiral motifs that occur in biomolecules, liquid crystals, ferroelectrics and antiferroelectrics, multiferroics, etc.

  4. Stationary and dispersive features in resonant inelastic soft X-ray scattering at the Ge 3p resonances

    Energy Technology Data Exchange (ETDEWEB)

    Glover, C.J. [Department of Electronic Materials Engineering, Australian National University, Canberra, ACT 0200 (Australia); Schmitt, T. [SLS, Paul Scherrer Institut, PSI West, CH-5232 Villigen PSI (Switzerland); Mattesini, M. [Departamento de Fisica de la Tierra, Astronomia y Astrofisica I, Universidad Complutense de Madrid, E-28040 (Spain); Adell, M.; Ilver, L.; Kanski, J. [Chalmers University of Technology, SE-412 96 Goeteborg (Sweden); Kjeldgaard, L. [MAX-lab, Lund University, P.O. Box 118, SE-22100 Lund (Sweden); Agaker, M. [Department of Physics and Materials Science, Uppsala University, PO Box 530, SE-751 21 Uppsala (Sweden); Martensson, N. [MAX-lab, Lund University, P.O. Box 118, SE-22100 Lund (Sweden); Department of Physics and Materials Science, Uppsala University, PO Box 530, SE-751 21 Uppsala (Sweden); Ahuja, R.; Nordgren, J. [Department of Physics and Materials Science, Uppsala University, PO Box 530, SE-751 21 Uppsala (Sweden); Rubensson, J.-E. [Department of Physics and Materials Science, Uppsala University, PO Box 530, SE-751 21 Uppsala (Sweden)], E-mail: jan-erik.rubensson@fysik.uu.se

    2009-07-15

    Resonant inelastic soft X-ray scattering at the 3p resonances in crystalline Ge is presented. Both stationary and dispersive features are observed in a wide energy range above as well as below the ionization limits. These observations are in agreement with theoretical predictions based on a two-step model where the initially excited electron has no influence on the emission step. Excess population of states in the conduction band is found, and discussed in terms of attosecond electron dynamics.

  5. An X-ray magnetic circular dichroism study of the interface Magnetism in titanate Heterostructures

    Science.gov (United States)

    Salluzzo, Marco; CNR-SPIN Team

    2014-03-01

    The 2D-electron system (2DES) created at the interface between LaAlO3 and SrTiO3 have attracted strong interest in recent years. This system shows an intriguing inversion the Ti3d bands hierarchy at the interface respect the bulk, and some reports even suggested coexistence between ferromagnetism and superconductivity. By using x-ray magnetic circular dichroism we show that oxygen vacancies induce magnetic interfacial localized Ti3 + states, which couple to the 2DES, with a negative exchange interaction. The magnetic dichroism signal is quenched in standard LAO/STO interfaces annealed in high oxygen pressure after the deposition and showing a homogeneous superconducting ground state, suggesting a decisive role of oxygen vacancies in the magnetism of these oxide interfaces.

  6. Probing the X-ray emission of old nulling pulsars with high magnetic fields

    Science.gov (United States)

    Posselt, Bettina

    2013-10-01

    We propose XMM-Newton observations of two nulling radio pulsars with magnetic fields B>10^(13)G. These long-period pulsars have spin-down properties, including characteristic ages, similar to those of the Magnificent Seven which are bright thermal X-ray emitters. Nulling pulsars have been suggested as evolutionary stage where the magnetospheric emission of a pulsar ceases. In contrast, no magnetospheric emission was detected at all at X-ray or radio wavelengths for the Magnificent Seven. The proposed XMM-Newton observations will probe the magneto-thermal NS evolution model as a potential link between the radio pulsar population and the Magnificent Seven. They will also provide for the first time an X-ray characterization of nulling pulsars with large magnetic fields.

  7. Determination of the magnetic fields of Magellanic X-ray pulsars

    Science.gov (United States)

    Christodoulou, Dimitris M.; Laycock, Silas G. T.; Yang, Jun; Fingerman, Samuel

    2017-05-01

    The 80 high-mass X-ray binary (HMXB) pulsars that are known to reside in the Magellanic Clouds (MCs) have been observed by the XMM-Newton and Chandra X-ray telescopes on a regular basis for 15 years, and the XMM-Newton and Chandra archives contain nearly complete information about the duty cycles of the sources with spin periods {P}{{S}}information about the magnitudes of their surface magnetic fields. We have found that the faintest states of the pulsars segregate into five discrete groups which obey to a high degree of accuracy the theoretical relation between spin period and X-ray luminosity. So the entire population of these pulsars can be described by just five propeller lines and the five corresponding magnetic moments (0.29, 0.53, 1.2, 2.9 and 7.3, in units of 1030 G cm3).

  8. Computational time-resolved and resonant x-ray scattering of strongly correlated materials

    Energy Technology Data Exchange (ETDEWEB)

    Bansil, Arun [Northeastern Univ., Boston, MA (United States)

    2016-11-09

    Basic-Energy Sciences of the Department of Energy (BES/DOE) has made large investments in x-ray sources in the U.S. (NSLS-II, LCLS, NGLS, ALS, APS) as powerful enabling tools for opening up unprecedented new opportunities for exploring properties of matter at various length and time scales. The coming online of the pulsed photon source, literally allows us to see and follow the dynamics of processes in materials at their natural timescales. There is an urgent need therefore to develop theoretical methodologies and computational models for understanding how x-rays interact with matter and the related spectroscopies of materials. The present project addressed aspects of this grand challenge of x-ray science. In particular, our Collaborative Research Team (CRT) focused on developing viable computational schemes for modeling x-ray scattering and photoemission spectra of strongly correlated materials in the time-domain. The vast arsenal of formal/numerical techniques and approaches encompassed by the members of our CRT were brought to bear through appropriate generalizations and extensions to model the pumped state and the dynamics of this non-equilibrium state, and how it can be probed via x-ray absorption (XAS), emission (XES), resonant and non-resonant x-ray scattering, and photoemission processes. We explored the conceptual connections between the time-domain problems and other second-order spectroscopies, such as resonant inelastic x-ray scattering (RIXS) because RIXS may be effectively thought of as a pump-probe experiment in which the incoming photon acts as the pump, and the fluorescent decay is the probe. Alternatively, when the core-valence interactions are strong, one can view K-edge RIXS for example, as the dynamic response of the material to the transient presence of a strong core-hole potential. Unlike an actual pump-probe experiment, here there is no mechanism for adjusting the time-delay between the pump and the probe. However, the core hole

  9. Magnetic soft x-ray microscopy of the domain wall depinning process in permalloy magnetic nanowires.

    Science.gov (United States)

    Im, Mi-Young; Bocklage, Lars; Meier, Guido; Fischer, Peter

    2012-01-18

    Full-field magnetic transmission x-ray microscopy at high spatial resolution down to 20 nm is used to directly observe field-driven domain wall motion in notch-patterned permalloy nanowires. The depinning process of a domain wall around a notch exhibits a stochastic nature in most nanowires. The stochasticity of the domain wall depinning sensitively depends on the geometry of the nanowire such as the wire thickness, the wire width, and the notch depth. We propose an optimized design of the nanowire for deterministic domain wall depinning field at a notch.

  10. A high-field pulsed magnet system for x-ray scattering studies in Voigt geometry

    CERN Document Server

    Islam, Zahirul; Ruff, Jacob P C; Das, Ritesh K; Trakhtenberg, Emil; Nojiri, Hiroyuki; Narumi, Yasuo; Canfield, Paul C

    2011-01-01

    We present a new pulsed-magnet system that enables x-ray single-crystal diffraction in addition to powder and spectroscopic studies in Voigt geometry. The apparatus consists of a large-bore solenoid, cooled by liquid nitrogen. A second independent closed-cycle cryostat is used for cooling samples near liquid helium temperatures. Pulsed magnetic fields up to ~30 T with a minimum of ~6 ms in total duration are generated by discharging a 40 kJ capacitor bank into the magnet coil. The unique characteristic of this instrument is the preservation of maximum scattering angle (~23.6 deg.) through the magnet bore by virtue of a novel double-funnel insert. This instrument would facilitate x-ray diffraction and spectroscopic studies that are impractical, if not impossible, to perform using conventional split-pair magnets and offers a practical solution for preserving optical access in future higher-field pulsed magnets.

  11. DEGRADATION OF MAGNET EPOXY AT NSLS X-RAY RING.

    Energy Technology Data Exchange (ETDEWEB)

    HU,J.P.; ZHONG,Z.; HAAS,E.; HULBERT,S.; HUBBARD,R.

    2004-05-24

    Epoxy resin degradation was analyzed for NSLS X-ring magnets after two decades of 2.58-2.8 GeV continuous electron-beam operation, based on results obtained from thermoluminescent dosimeters irradiated along the NSLS ring and epoxy samples irradiated at the beamline target location. A Monte Carlo-based particle transport code, MCNP, was utilized to verify the dose from synchrotron radiation distributed along the axial- and transverse-direction in a ring model, which simulates the geometry of a ring quadrupole magnet and its central vacuum chamber downstream of the bending-magnet photon ports. The actual life expectancy of thoroughly vacuum baked-and-cured epoxy resin was estimated from radiation tests on similar polymeric materials using a radiation source developed for electrical insulation and mechanical structure studies.

  12. Extreme ultraviolet resonant inelastic X-ray scattering (RIXS) at a seeded free-electron laser

    Science.gov (United States)

    Dell’Angela, M.; Hieke, F.; Malvestuto, M.; Sturari, L.; Bajt, S.; Kozhevnikov, I. V.; Ratanapreechachai, J.; Caretta, A.; Casarin, B.; Glerean, F.; Kalashnikova, A. M.; Pisarev, R. V.; Chuang, Y.-D.; Manzoni, G.; Cilento, F.; Mincigrucci, R.; Simoncig, A.; Principi, E.; Masciovecchio, C.; Raimondi, L.; Mahne, N.; Svetina, C.; Zangrando, M.; Passuello, R.; Gaio, G.; Prica, M.; Scarcia, M.; Kourousias, G.; Borghes, R.; Giannessi, L.; Wurth, W.; Parmigiani, F.

    2016-12-01

    In the past few years, we have been witnessing an increased interest for studying materials properties under non-equilibrium conditions. Several well established spectroscopies for experiments in the energy domain have been successfully adapted to the time domain with sub-picosecond time resolution. Here we show the realization of high resolution resonant inelastic X-ray scattering (RIXS) with a stable ultrashort X-ray source such as an externally seeded free electron laser (FEL). We have designed and constructed a RIXS experimental endstation that allowed us to successfully measure the d-d excitations in KCoF3 single crystals at the cobalt M2,3-edge at FERMI FEL (Elettra-Sincrotrone Trieste, Italy). The FEL-RIXS spectra show an excellent agreement with the ones obtained from the same samples at the MERIXS endstation of the MERLIN beamline at the Advanced Light Source storage ring (Berkeley, USA). We established experimental protocols for performing time resolved RIXS experiments at a FEL source to avoid X ray-induced sample damage, while retaining comparable acquisition time to the synchrotron based measurements. Finally, we measured and modelled the influence of the FEL mixed electromagnetic modes, also present in externally seeded FELs, and the beam transport with ~120 meV experimental resolution achieved in the presented RIXS setup.

  13. Trends in ultracool dwarf magnetism. I. X-ray suppression and radio enhancement

    Energy Technology Data Exchange (ETDEWEB)

    Williams, P. K. G.; Berger, E. [Harvard-Smithsonian Center for Astrophysics, 60 Garden Street, Cambridge, MA 02138 (United States); Cook, B. A., E-mail: pwilliams@cfa.harvard.edu [Department of Astrophysical Sciences, Princeton University, Princeton, NJ 08544 (United States)

    2014-04-10

    Although ultracool dwarfs (UCDs) are now known to generate and dissipate strong magnetic fields, a clear understanding of the underlying dynamo is still lacking. We have performed X-ray and radio observations of seven UCDs in a narrow range of spectral type (M6.5-M9.5) but spanning a wide range of projected rotational velocities (vsin i ≈ 3-40 km s{sup –1}). We have also analyzed unpublished archival Chandra observations of four additional objects. All of the newly observed targets are detected in the X-ray, while only one is detected in the radio, with the remainder having sensitive upper limits. We present a database of UCDs with both radio and X-ray measurements and consider the data in light of the so-called Güdel-Benz relation (GBR) between magnetic activity in these bands. Some UCDs have very bright radio emission and faint X-ray emission compared to what would be expected for rapid rotators, while others show the opposite behavior. We show that UCDs would still be radio-overluminous relative to the GBR even if their X-ray emission were at standard rapid-rotator 'saturation' levels. Recent results from Zeeman-Doppler imaging and geodynamo simulations suggest that rapidly rotating UCDs may harbor a bistable dynamo that supports either a stronger, axisymmetric magnetic field or a weaker, non-axisymmetric field. We suggest that the data can be explained in a scenario in which strong-field objects obey the GBR while weak-field objects are radio-overluminous and X-ray-underluminous, possibly because of a population of gyrosynchrotron-emitting coronal electrons that is continuously replenished by low-energy reconnection events.

  14. Population Inversion and Gain Measurements for Soft X-Ray Laser Development in a Magnetically Confined Plasma Column.

    Science.gov (United States)

    1985-09-01

    INVERSION AND GAIN MEASUREMENTS FOR ’I SOFT X-RAY LASER DEVELOPMENT IN A MAGNET ICALLY CONFINED PLASMA COLUMN" For the Period: Nov. 1, 1983 t hr u Sept...proposal to AFOSR entitled "Population Inversion and Gain Measurements for X-Ray Laser Development in Magnetically Confined Plasma Column," Princeton, March...I* INTRODUCTION Extensive research on x-ray laser development has provided a number of interesting results for different schemes, e.g. recombination

  15. Standing-wave excited soft x-ray photoemission microscopy: application to Co microdot magnetic arrays

    Energy Technology Data Exchange (ETDEWEB)

    Gray, Alexander; Kronast, Florian; Papp, Christian; Yang, See-Hun; Cramm, Stefan; Krug, Ingo P.; Salmassi, Farhad; Gullikson, Eric M.; Hilken, Dawn L.; Anderson, Erik H.; Fischer, Peter; Durr, Hermann A.; Schneider, Claus M.; Fadley, Charles S.

    2010-10-29

    We demonstrate the addition of depth resolution to the usual two-dimensional images in photoelectron emission microscopy (PEEM), with application to a square array of circular magnetic Co microdots. The method is based on excitation with soft x-ray standing-waves generated by Bragg reflection from a multilayer mirror substrate. Standing wave is moved vertically through sample simply by varying the photon energy around the Bragg condition. Depth-resolved PEEM images were obtained for all of the observed elements. Photoemission intensities as functions of photon energy were compared to x-ray optical calculations in order to quantitatively derive the depth-resolved film structure of the sample.

  16. Highly charged ion X-rays from Electron-Cyclotron Resonance Ion Sources

    OpenAIRE

    Indelicato, Paul; Boucard, S.; Covita, D. S.; Gotta, D.; Gruber, A; Hirtl, A.; Fuhrmann, H.; Le Bigot, E.-O.; Schlesser, S.; dos Santos, J. M. F.; Simons, L.M.; Stingelin, L.; Trassinelli, Martino; Veloso, J.; Wasser, A.

    2006-01-01

    Radiation from the highly-charged ions contained in the plasma of Electron-Cyclotron Resonance Ion Sources constitutes a very bright source of X-rays. Because the ions have a relatively low kinetic energy ($\\approx 1$~eV) transitions can be very narrow, containing only small Doppler broadening. We describe preliminary accurate measurements of two and three-electron ions with $Z=16$--18. We show how these measurement can test sensitively many-body relativistic calculations or can be used as X-...

  17. Novel rhenium gasket design for nuclear resonant inelastic x-ray scattering at high pressure.

    Science.gov (United States)

    Tanis, Elizabeth A; Giefers, Hubertus; Nicol, Malcolm F

    2008-02-01

    For the first time, a highly absorbing element, rhenium, has been proven to be a strong, reliable, and safe gasket material for achieving high pressure in nuclear resonant inelastic x-ray scattering (NRIXS) experiments. Rhenium foil was cut into rectangular slices and in order to reduce absorption, the elevated imprint due to preindenting of the gasket is removed using electrical discharge machining. By utilizing this novel gasket design, transmission losses were mitigated while performing NRIXS experiments conducted on the 119Sn and 57Fe Mössbauer isotopes.

  18. Local X-ray magnetic circular dichroism study of Fe/Cu(111) using a tunneling smart tip

    Energy Technology Data Exchange (ETDEWEB)

    DiLullo, Andrew; Shirato, Nozomi; Cummings, Marvin [Argonne National Laboratory, 9700 South Cass Avenue, Argonne, IL 60439 (United States); Kersell, Heath; Chang, Hao [Argonne National Laboratory, 9700 South Cass Avenue, Argonne, IL 60439 (United States); Ohio University, Athens, OH 45701 (United States); Rosenmann, Daniel; Miller, Dean; Freeland, John W. [Argonne National Laboratory, 9700 South Cass Avenue, Argonne, IL 60439 (United States); Hla, Saw-Wai [Argonne National Laboratory, 9700 South Cass Avenue, Argonne, IL 60439 (United States); Ohio University, Athens, OH 45701 (United States); Rose, Volker, E-mail: vrose@anl.gov [Argonne National Laboratory, 9700 South Cass Avenue, Argonne, IL 60439 (United States); Argonne National Laboratory, 9700 South Cass Avenue, Argonne, IL 60439 (United States)

    2016-01-28

    A tunneling smart tip of a synchrotron X-ray scanning tunneling microscope provides simultaneously localized topographic, elemental and magnetic information. Localized spectroscopy with simultaneous topographic, elemental and magnetic information is presented. A synchrotron X-ray scanning tunneling microscope has been employed for the local study of the X-ray magnetic circular dichroism at the Fe L{sub 2,3}-edges of a thin iron film grown on Cu(111). Polarization-dependent X-ray absorption spectra have been obtained through a tunneling smart tip that serves as a photoelectron detector. In contrast to conventional spin-polarized scanning tunneling microscopy, X-ray excitations provide magnetic contrast even with a non-magnetic tip. Intensity variations in the photoexcited tip current point to chemical variations within a single magnetic Fe domain.

  19. Low-energy d-d excitations in MnO studied by resonant x-ray fluorescence spectroscopy

    Energy Technology Data Exchange (ETDEWEB)

    Butorin, S.M.; Guo, J.; Magnuson, M. [Uppsala Univ. (Sweden)] [and others

    1997-04-01

    Resonant soft X-ray emission spectroscopy has been demonstrated to possess interesting abilities for studies of electronic structure in various systems, such as symmetry probing, alignment and polarization dependence, sensitivity to channel interference, etc. In the present abstract the authors focus on the feasibility of resonant soft X-ray emission to probe low energy excitations by means of resonant electronic X-ray Raman scattering. Resonant X-ray emission can be regarded as an inelastic scattering process where a system in the ground state is transferred to a low excited state via a virtual core excitation. The energy closeness to a core excitation of the exciting radiation enhances the (generally) low probability for inelastic scattering at these wavelengths. Therefore soft X-ray emission spectroscopy (in resonant electronic Raman mode) can be used to study low energy d-d excitations in transition metal systems. The involvement of the intermediate core state allows one to use the selection rules of X-ray emission, and the appearance of the elastically scattered line in the spectra provides the reference to the ground state.

  20. Minimalist coupled evolution model for stellar x-ray activity, rotation, mass loss, and magnetic field

    CERN Document Server

    Blackman, Eric G

    2015-01-01

    Late-type main sequence stars exhibit an x-ray to bolometric flux that depends on the Corolis number $Co$ (product of convective turnover time and angular rotation speed) as $Co^{\\zeta}$ with $2\\le \\zeta \\le 3$ for $Co > 1$. Stars in the unsaturated regime also obey the Skumanich law--- their rotation speeds scale inversely with square root of their age. The associated stellar magnetic field strengths follow a similar decrease with age. While the connection between faster rotators, stronger fields, and higher activity has been well established observationally, a basic theory for the time evolution of x-ray luminosity, rotation, magnetic field and mass loss been lacking. Here we offer a minimalist model for the time evolution of these quantities built from combining a Parker wind with several new ingredients: (1) explicit sourcing of both the thermal energy launching the wind and the x-ray luminosity via dynamo produced magnetic fields; (2) explicit coupling of x-ray activity and mass loss saturation to dynamo...

  1. Mössbauer, magnetization and X-ray diffraction characterization methods for iron oxide nanoparticles

    Energy Technology Data Exchange (ETDEWEB)

    Gabbasov, Raul, E-mail: gabbasov-raul@yandex.ru [National Research Center “Kurchatov Institute”, Moscow (Russian Federation); Polikarpov, Michael; Cherepanov, Valery [National Research Center “Kurchatov Institute”, Moscow (Russian Federation); Chuev, Michael; Mischenko, Iliya; Lomov, Andrey [Institute of Physics and Technology, Russian Academy of Sciences, Moscow (Russian Federation); Wang, Andrew [Ocean NanoTech. Springdale, AR (United States); Panchenko, Vladislav [National Research Center “Kurchatov Institute”, Moscow (Russian Federation)

    2015-04-15

    Water soluble magnetite iron oxide nanoparticles with oleic polymer coating and average diameters in the range of 5–25 nm, previously determined by TEM, were characterized using Mössbauer, magnetization and X-ray diffraction measurements. Comparative analysis of the results demonstrated a large diversity of magnetic relaxation regimes. Analysis showed the presence of an additional impurity component in the 25 nm nanoparticles, with principally different magnetic nature at the magnetite core. In some cases, X-ray diffraction measurements were unable to estimate the size of the magnetic core and Mössbauer data were necessary for the correct interpretation of the experimental results. - Highlights: • KV parameter, obtained from Mössbauer spectra can be used for nanoparticle size characterization. • Mössbauer spectra of 10–25 nm nanoparticles can be effectively described by ferromagnetic model. • Surface impurities can cause incorrect nanoparticle size determination.

  2. Investigating the electron density of multi-MeV X-ray-induced air plasmas at low pressures based on electromagnetic resonant cavity analysis

    Science.gov (United States)

    Ribière, M.; d'Almeida, T.; Cessenat, O.; Maulois, M.; Pouzalgues, R.; Crabos, B.; Delbos, C.; Garrigues, A.; Azaïs, B.

    2016-12-01

    We investigate air plasmas generated by multi-MeV pulsed X-rays at pressures ranging from 10-5 to 10-1 mbar. The experimental approach used for these studies is based on measurements of resonant frequencies damping and shift for different electromagnetic modes within a cylindrical cavity. Time-integrated electron densities in X-ray-induced air plasmas are inferred from the damping rate of the measured magnetic fields and their corresponding frequency shifts. In the present study, electron densities ranging from 108 to 109 cm-3 at pressures ranging from 10-3 to 10-1 mbar have been measured. Experimental results were confronted to 3D Maxwell-Vlasov Particle-In-Cell simulations incorporating a radiation-induced electric conductivity model. The method used in this work enables determining microscopic and macroscopic physical quantities within low pressure air plasmas generated by pulsed X-ray.

  3. Calculations of magnetic x-ray dichroism in the 3d absorption spectra of rare-earth compounds

    NARCIS (Netherlands)

    GOEDKOOP, JB; THOLE, BT; VANDERLAAN, G; SAWATZKY, GA; DEGROOT, FMF; FUGGLE, JC; de Groot, Frank

    1988-01-01

    We present atomic calculations for the recently discovered magnetic x-ray dichroism (MXD) displayed by the 3d x-ray-absorption spectra of rare-earth compounds. The spectral shapes expected at T=0 K for linear polarization parallel and normal to the local magnetic field is given, together with the te

  4. X-ray MCD Measurements in a high Tc molecular-based magnet

    NARCIS (Netherlands)

    Arrio, M.-A.; Sainctavit, Ph.; Cartier dit Moulin, Ch.; Brouder, Ch.; Groot, F.M.F. de; Mallah, T.; Verdaguer, M.

    1996-01-01

    The molecular based magnet Cs^(I)[Ni^(II)Cr^(III)(CN)6]. 2H2O is a ferromagnet with a Curie temperature Tc = 90 K. Its structure consists of face centred cubic lattice of Ni^(II) ions connected by Cr(CN)6 entities. We have recorded X-ray Magnetic Circular Dichroism (XMCD) at nickel L2,3 edges. It

  5. X-ray MCD Measurements in a high Tc molecular-based magnet

    NARCIS (Netherlands)

    Arrio, M.-A.; Sainctavit, Ph.; Cartier dit Moulin, Ch.; Brouder, Ch.; Groot, F.M.F. de; Mallah, T.; Verdaguer, M.

    2001-01-01

    The molecular based magnet Cs^(I)[Ni^(II)Cr^(III)(CN)6]. 2H2O is a ferromagnet with a Curie temperature Tc = 90 K. Its structure consists of face centred cubic lattice of Ni^(II) ions connected by Cr(CN)6 entities. We have recorded X-ray Magnetic Circular Dichroism (XMCD) at nickel L2,3 edges. It cl

  6. X-ray magnetic circular dichroism in Co2FeGa: First-principles calculations

    Science.gov (United States)

    Kukusta, D. A.; Antonov, V. N.; Yaresko, A. N.

    2011-08-01

    The electronic structure and x-ray magnetic circular dichroism (XMCD) spectra of the Heusler alloy Co2FeGa were investigated theoretically from first principles, using the fully relativistic Dirac linear MT-orbital (LMTO) band structure method. Densities of valence states, orbital and spin magnetic moments are analyzed and discussed. The origin of the XMCD spectra in the Co2FeGa compound is examined. The calculated results are compared with available experimental data.

  7. Soft X-ray Resonant Scattering in Manganites as a Probe of Orbital Order: Theoretical Predictions

    Science.gov (United States)

    Altarelli, Massimo

    2001-03-01

    The claim of the detection of orbital order [1] in manganites by resonant x-ray scattering at the Mn K-edge has raised considerable controversy [2] because of the indirect mechanism by which properties of the 3d electrons are probed by a process involving excitation into the 4p states. In particular, the possibility that x-ray experiments probe Jahn-Teller displacements, rather than orbital order, has been debated. An alternative proposal [3] is to use resonant scattering at the Mn L2 and L3 edges, with dipole allowed excitation into 3d states, as a more direct probe allowing to separate effects related to the order of the 3d orbitals from lattice displacements. Given the longer wavelength, only order with a period longer than about 0.97 nm is accessible. There are however systems, like La_1-x(Ca,Sr)_xMnO3 for x=0.5, x=0.33, etc., in addition to La_0.5Sr_1.5MnO4 where this condition is fulfilled. Calculations within an atomic multiplet scheme, with inclusion of crystal field effects, which point to an easier separation of orbital order from lattice displacements in the soft x-ray case, are presented and discussed. Different structures in the energy dependence of the scattering intensity are related predominantly to one of the two mechanisms. Other issues, such as the smaller scattering volume due to photoelectric absorption effects, are also addressed. 1. Y. Murakami et al., Phys. Rev. Lett. 80, 1932 (1998); ibid. 81, 582 (1998). 2. Elfimov et al., Phys. Rev. Lett. 82, 4264 (1998); M. Benfatto et al., Phys. Rev. Lett. 83, 636 (1999); M. Takahashi et al., J. Phys. Soc. Japan 68, 2530 (1999). 3. C.W.M. Castleton and M. Altarelli, Phys. Rev B 62, 1033 (2000).

  8. Interplay between relativistic energy corrections and resonant excitations in x-ray multiphoton ionization dynamics of Xe atoms

    Science.gov (United States)

    Toyota, Koudai; Son, Sang-Kil; Santra, Robin

    2017-04-01

    In this paper, we theoretically study x-ray multiphoton ionization dynamics of heavy atoms taking into account relativistic and resonance effects. When an atom is exposed to an intense x-ray pulse generated by an x-ray free-electron laser (XFEL), it is ionized to a highly charged ion via a sequence of single-photon ionization and accompanying relaxation processes, and its final charge state is limited by the last ionic state that can be ionized by a single-photon ionization. If x-ray multiphoton ionization involves deep inner-shell electrons in heavy atoms, energy shifts by relativistic effects play an important role in ionization dynamics, as pointed out in Phys. Rev. Lett. 110, 173005 (2013), 10.1103/PhysRevLett.110.173005. On the other hand, if the x-ray beam has a broad energy bandwidth, the high-intensity x-ray pulse can drive resonant photoexcitations for a broad range of ionic states and ionize even beyond the direct one-photon ionization limit, as first proposed in Nat. Photon. 6, 858 (2012), 10.1038/nphoton.2012.261. To investigate both relativistic and resonance effects, we extend the xatom toolkit to incorporate relativistic energy corrections and resonant excitations in x-ray multiphoton ionization dynamics calculations. Charge-state distributions are calculated for Xe atoms interacting with intense XFEL pulses at a photon energy of 1.5 keV and 5.5 keV, respectively. For both photon energies, we demonstrate that the role of resonant excitations in ionization dynamics is altered due to significant shifts of orbital energy levels by relativistic effects. Therefore, it is necessary to take into account both effects to accurately simulate multiphoton multiple ionization dynamics at high x-ray intensity.

  9. X-ray emission from star-forming galaxies - signatures of cosmic rays and magnetic fields

    Science.gov (United States)

    Schober, J.; Schleicher, D. R. G.; Klessen, R. S.

    2015-01-01

    The evolution of magnetic fields in galaxies is still an open problem in astrophysics. In nearby galaxies the far-infrared-radio correlation indicates the coupling between magnetic fields and star formation. The correlation arises from the synchrotron emission of cosmic ray electrons travelling through the interstellar magnetic fields. However, with an increase of the interstellar radiation field (ISRF), inverse Compton scattering becomes the dominant energy loss mechanism of cosmic ray electrons with a typical emission frequency in the X-ray regime. The ISRF depends on the one hand on the star formation rate and becomes stronger in starburst galaxies, and on the other hand increases with redshift due to the higher temperature of the cosmic microwave background. With a model for the star formation rate of galaxies, the ISRF, and the cosmic ray spectrum, we can calculate the expected X-ray luminosity resulting from the inverse Compton emission. Except for galaxies with an active galactic nucleus the main additional contribution to the X-ray luminosity comes from X-ray binaries. We estimate this contribution with an analytical model as well as with an observational relation, and compare it to the pure inverse Compton luminosity. Using data from the Chandra Deep Field Survey and far-infrared observations from Atacama Large Millimeter/Submillimeter Array, we then determine upper limits for the cosmic ray energy. Assuming that the magnetic energy in a galaxy is in equipartition with the energy density of the cosmic rays, we obtain upper limits for the magnetic field strength. Our results suggest that the mean magnetic energy of young galaxies is similar to the one in local galaxies. This points towards an early generation of galactic magnetic fields, which is in agreement with current dynamo evolution models.

  10. Trends in Ultracool Dwarf Magnetism. I. X-Ray Suppression and Radio Enhancement

    CERN Document Server

    Williams, P K G; Berger, E

    2013-01-01

    Although ultracool dwarfs (UCDs) are now known to generate and dissipate strong magnetic fields, a clear understanding of the underlying dynamo is still lacking. We have performed X-ray and radio observations of seven UCDs in a narrow range of spectral type (M6.5-M9.5) but spanning a wide range of projected rotational velocities (v sin i ~ 3-40 km/s). We have also analyzed unpublished archival Chandra observations of four additional objects. All of the newly-observed targets are detected in the X-ray, while only one is detected in the radio, with the remainder having sensitive upper limits. We present a database of UCDs with both radio and X-ray measurements and consider the data in light of the so-called G\\"udel-Benz relation (GBR) between magnetic activity in these bands. Some UCDs have very bright radio emission and faint X-ray emission compared to what would be expected for rapid rotators, while others show opposite behavior. We show that UCDs would still be radio-over-luminous relative to the GBR even if...

  11. Identification of inversion domains in KTiOPO4 via resonant X-ray diffraction.

    Science.gov (United States)

    Fabrizi, Federica; Thomas, Pamela A; Nisbet, Gareth; Collins, Stephen P

    2015-07-01

    A novel method is presented for the identification of the absolute crystallographic structure in multi-domain polar materials such as ferroelectric KTiOPO4. Resonant (or 'anomalous') X-ray diffraction spectra collected across the absorption K edge of Ti (4.966 keV) on a single Bragg reflection demonstrate a huge intensity ratio above and below the edge, providing a polar domain contrast of ∼270. This allows one to map the spatial domain distribution in a periodically inverted sample, with a resolution of ∼1 µm achieved with a microfocused beam. This non-contact, non-destructive technique is well suited for samples of large dimensions (in contrast with traditional resonant X-ray methods based on diffraction from Friedel pairs), and its potential is particularly relevant in the context of physical phenomena connected with an absence of inversion symmetry, which require characterization of the underlying absolute atomic structure (such as in the case of magnetoelectric coupling and multiferroics).

  12. Femtosecond Single-Shot Imaging of Nanoscale Ferromagnetic Order in Co/Pd Multilayers using Resonant X-ray Holography

    Energy Technology Data Exchange (ETDEWEB)

    Wang, Tianhan; Zhu, Diling; Benny Wu,; Graves, Catherine; Schaffert, Stefan; Rander, Torbjorn; Muller, leonard; Vodungbo, Boris; Baumier, Cedric; Bernstein, David P.; Brauer, Bjorn; Cros, Vincent; Jong, Sanne de; Delaunay, Renaud; Fognini, Andreas; Kukreja, Roopali; Lee, Sooheyong; Lopez-Flores, Victor; Mohanty, Jyoti; Pfau, Bastian; Popescu, 5 Horia

    2012-05-15

    We present the first single-shot images of ferromagnetic, nanoscale spin order taken with femtosecond x-ray pulses. X-ray-induced electron and spin dynamics can be outrun with pulses shorter than 80 fs in the investigated fluence regime, and no permanent aftereffects in the samples are observed below a fluence of 25 mJ/cm{sup 2}. Employing resonant spatially-muliplexed x-ray holography results in a low imaging threshold of 5 mJ/cm{sup 2}. Our results open new ways to combine ultrafast laser spectroscopy with sequential snapshot imaging on a single sample, generating a movie of excited state dynamics.

  13. Why are millisecond pulsar magnetic fields low and how do their X-rays arise?

    Science.gov (United States)

    Webb, Natalie

    2006-10-01

    Binary millisecond pulsars (MSPs) found in the field are thought to be recycled from accreting pulsars. These MSPs have short periods, low spindown rates (Pdot) and consequently low surface magnetic fields (Bs) as Bs is proportional to (Pdot P)^0.5. It is unclear, however, how the MSP surface magnetic field can evolve from the high fields observed in pulsars to the low MSP values. Two models have been proposed to explain this. Also, the origin of the high energy emission is unclear as too few MSP X-ray observations have been made to differentiate between competing models. With these XMM-Newton observations of four MSPs previously unobserved in X-rays, we will discriminate between differing models describing the magnetic field evolution and the high energy emission origin.

  14. X-Ray Emission from Star-Forming Galaxies - Signatures of Cosmic Rays and Magnetic Fields

    CERN Document Server

    Schober, Jennifer; Klessen, Ralf S

    2014-01-01

    The evolution of magnetic fields in galaxies is still an open problem in astrophysics. In nearby galaxies the far-infrared-radio correlation indicates the coupling between magnetic fields and star formation. The correlation arises from the synchrotron emission of cosmic ray electrons traveling through the interstellar magnetic fields. However, with an increase of the interstellar radiation field (ISRF), inverse Compton scattering becomes the dominant energy loss mechanism of cosmic ray electrons with a typical emission frequency in the X-ray regime. The ISRF depends on the one hand on the star formation rate and becomes stronger in starburst galaxies, and on the other hand increases with redshift due to the evolution of the cosmic microwave background. With a model for the star formation rate of galaxies, the ISRF, and the cosmic ray spectrum, we can calculate the expected X-ray luminosity resulting from the inverse Compton emission. Except for galaxies with an active galactic nucleus the main additional cont...

  15. Characterization and Performance of Magnetic Calorimeters for Applications in X-ray Spectroscopy

    Science.gov (United States)

    Porst, J.-P.; Bandler, S. R.; Adams, J. S.; Balvin, M. A.; Busch, S. E.; Eckart, M. E.; Kelley, R. L.; Kilbourne, C. A.; Lee, S. J.; Nagler, P. C.; Porter, F. S.; Sadleir, J. E.; Seidel, G. M.; Smith, S. J.; Stevenson, T. R.

    2014-09-01

    We have developed prototype arrays of metallic magnetic calorimeters for applications in X-ray astronomy. Each pixel consists of an all-gold X-ray absorber in good thermal contact to a gold-erbium paramagnetic thin film thermometer that is operated in the temperature range of 30-100 mK. The para-magnetic response is coupled to a SQUID amplifier. We have characterized pixels in an array and observed the expected temperature dependence of the magnetization and heat capacity. We have demonstrated a full width at half maximum energy resolution of 1.7 0.1 eV at 6 keV and have also read out these devices using time-division multiplexing.

  16. X-ray Detection of Transient Magnetic Moments Induced by a Spin Current in Cu.

    Science.gov (United States)

    Kukreja, R; Bonetti, S; Chen, Z; Backes, D; Acremann, Y; Katine, J A; Kent, A D; Dürr, H A; Ohldag, H; Stöhr, J

    2015-08-28

    We have used a MHz lock-in x-ray spectromicroscopy technique to directly detect changes in magnetic moment of Cu due to spin injection from an adjacent Co layer. The elemental and chemical specificity of x rays allows us to distinguish two spin current induced effects. We detect the creation of transient magnetic moments of 3×10^{-5}μ_{B} on Cu atoms within the bulk of the 28 nm thick Cu film due to spin accumulation. The moment value is compared to predictions by Mott's two current model. We also observe that the hybridization induced existing magnetic moments at the Cu interface atoms are transiently increased by about 10% or 4×10^{-3}μ_{B} per atom. This reveals the dominance of spin-torque alignment over Joule heat induced disorder of the interfacial Cu moments during current flow.

  17. X-ray detection of transient magnetic moments induced by a spin current in Cu

    Energy Technology Data Exchange (ETDEWEB)

    Kukreja, R. [SLAC National Accelerator Lab., Menlo Park, CA (United States); Stanford Univ., Stanford, CA (United States); Bonetti, S. [SLAC National Accelerator Lab., Menlo Park, CA (United States); Stanford Univ., Stanford, CA (United States); Chen, Z. [SLAC National Accelerator Lab., Menlo Park, CA (United States); Stanford Univ., Stanford, CA (United States); Backes, D. [New York Univ. (NYU), New York, NY (United States); Acremann, Y. [ETH Zurich, Zurich (Switzerland); Katine, J. [HGST, a Western Digital Company, San Jose, CA (United States); Kent, A. D. [New York Univ. (NYU), New York, NY (United States); Durr, H. A. [SLAC National Accelerator Lab., Menlo Park, CA (United States); Ohldag, H. [SLAC National Accelerator Lab., Menlo Park, CA (United States); Stohr, J. [SLAC National Accelerator Lab., Menlo Park, CA (United States)

    2015-08-24

    We have used a MHz lock-in x-ray spectromicroscopy technique to directly detect changes in magnetic moment of Cu due to spin injection from an adjacent Co layer. The elemental and chemical specificity of x rays allows us to distinguish two spin current induced effects. We detect the creation of transient magnetic moments of 3×10–5μB on Cu atoms within the bulk of the 28 nm thick Cu film due to spin accumulation. The moment value is compared to predictions by Mott’s two current model. We also observe that the hybridization induced existing magnetic moments at the Cu interface atoms are transiently increased by about 10% or 4×10–3μB per atom. As a result, this reveals the dominance of spin-torque alignment over Joule heat induced disorder of the interfacial Cu moments during current flow.

  18. Soft gamma-ray repeaters and anomalous X-ray pulsars as highly magnetized white dwarfs

    CERN Document Server

    Mukhopadhyay, Banibrata

    2016-01-01

    We show that the soft gamma-ray repeaters (SGRs) and anomalous X-ray pulsars (AXPs) can be explained as recently proposed highly magnetized white dwarfs (B-WDs). The radius and magnetic field of B-WDs are perfectly adequate to explain energies in SGRs/AXPs as the rotationally powered energy. While the highly magnetized neutron stars require an extra, observationally not well established yet, source of energy, the magnetized white dwarfs, yet following Chandrasekhar's theory (C-WDs), exhibit large ultra-violet luminosity which is observationally constrained from a strict upper limit.

  19. The simultaneous measurement of energy and linear polarization of the scattered radiation in resonant inelastic soft x-ray scattering

    Energy Technology Data Exchange (ETDEWEB)

    Braicovich, L., E-mail: lucio.braicovich@polimi.it; Minola, M.; Dellea, G.; Ghiringhelli, G. [CNR-SPIN and Dipartimento di Fisica, Politecnico di Milano, piazza Leonardo Da Vinci 32, Milano I-20133 (Italy); Le Tacon, M. [Max-Planck-Institut für Festkörperforschung, Heisenbergstrasse 1, D-70569 Stuttgart (Germany); Moretti Sala, M.; Morawe, C.; Peffen, J.-Ch.; Yakhou, F.; Brookes, N. B. [European Synchrotron Radiation Facility, 71 Avenue des Martyrs, Grenoble F-38043 (France); Supruangnet, R. [Synchrotron Light Research Institute, Nakhon Ratchasima (Thailand)

    2014-11-15

    Resonant Inelastic X-ray Scattering (RIXS) in the soft x-ray range is an element-specific energy-loss spectroscopy used to probe the electronic and magnetic excitations in strongly correlated solids. In the recent years, RIXS has been progressing very quickly in terms of energy resolution and understanding of the experimental results, but the interpretation of spectra could further improve, sometimes decisively, from a full knowledge of the polarization of incident and scattered photons. Here we present the first implementation, in a high resolution soft-RIXS spectrometer used to analyze the scattered radiation, of a device allowing the measurement of the degree of linear polarization. The system, based on a graded W/B{sub 4}C multilayer mirror installed in proximity of the CCD detector, has been installed on the AXES spectrometer at the ESRF (European Synchrotron Radiation Facility); it has been fully characterized and it has been used for a demonstration experiment at the Cu L{sub 3} edge on a high-T{sub c} superconducting cuprate. The loss in efficiency suffered by the spectrometer equipped with this test facility was a factor 17.5. We propose also a more advanced version, suitable for a routine use on the next generation of RIXS spectrometers and with an overall efficiency up to 10%.

  20. The simultaneous measurement of energy and linear polarization of the scattered radiation in resonant inelastic soft x-ray scattering

    CERN Document Server

    Braicovich, L; Dellea, G; Tacon, M Le; Sala, M Moretti; Morawe, C; Peffen, J-Ch; Supruangnet, R; Yakhou, F; Ghiringhelli, G; Brookes, N B

    2014-01-01

    Resonant Inelastic X-ray Scattering (RIXS) in the soft x-ray range is an element-specific energy-loss spectroscopy used to probe the electronic and magnetic excitations in strongly correlated solids. In the recent years, RIXS has been progressing very quickly in terms of energy resolution and understanding of the experimental results, but the interpretation of spectra could further improve, sometimes decisively, from a full knowledge of the polarization of incident and scattered photons. Here we present the first implementation, in a high resolution RIXS spectrometer used to analyze the scattered radiation, of a device allowing the measurement of the degree of linear polarization. The system, based on a graded W/B4C multilayer mirror installed in proximity of the CCD detector, has been installed on the AXES spectrometer at the ESRF; it has been fully characterized and it has been used for a demonstration experiment at the Cu L3 edge on a high-Tc superconducting cuprate. The loss in efficiency suffered by the ...

  1. Modality-integrated magnetic catheter tracking for x-ray vascular interventions

    Energy Technology Data Exchange (ETDEWEB)

    Krueger, Sascha [Philips Research Laboratories, Division Technical Systems, Roentgenstrasse 24-26, 22335 Hamburg (Germany); Timinger, Holger [Philips Research Laboratories, Division Technical Systems, Roentgenstrasse 24-26, 22335 Hamburg (Germany); Grewer, Ruediger [Philips Research Laboratories, Division Technical Systems, Roentgenstrasse 24-26, 22335 Hamburg (Germany); Borgert, Joern [Philips Research Laboratories, Division Technical Systems, Roentgenstrasse 24-26, 22335 Hamburg (Germany)

    2005-02-21

    A novel setup for the integration of a magnetic tracking system (MTS) into a catheter laboratory environment by attaching the field generator of the MTS to the C-arm of the x-ray system was investigated. The metal interference of the x-ray system with the MTS then becomes static and can be calibrated. The registration of a tracked catheter to 2D live x-ray images with high and well-defined accuracy is thus possible for arbitrary C-arm positions. Interference with imaging by blocking the field of view is avoided. Real-time registration methods to maintain the registration of the catheter also to static 2D or 3D images (roadmaps), regardless of the C-arm rotation during catheter tracking, were investigated. Residual registration errors of the tracked catheter with respect to the static roadmaps (2D and 3D) were reduced by using the vessel geometry and shape information. The algorithms potentially allow for motion correction (e.g. due to respiration). Using the shape-based correction algorithms the average registration accuracies to static roadmaps for different C-arm angulations and catheter positions were determined to be 3.3-4.2 mm. The magnetic registration of the C-arm was furthermore allowed to compute the imaging geometry (position of the C-arm) and to produce virtual angiographic preview images before contrast injection and x-ray dose application. Thus, optimal projection geometries and collimator settings for the target region can be chosen in an 'off line' fashion. The proposed MTS-supported navigation setup on both 3D (static) and 2D (live and static) roadmaps merges the high resolution and real-time feedback of 2D x-ray images with the navigation support from 3D static images.

  2. A new model for the X-ray continuum of the magnetized accreting pulsars

    CERN Document Server

    Farinelli, R; Bozzo, E; Becker, P A

    2016-01-01

    Accreting highly magnetized pulsars in binary systems are among the brightest X-ray emitters in our Galaxy. Although a number of high statistical quality broad-band (0.1-100 keV) X-ray observations are available, the spectral energy distribution of these sources is usually investigated by adopting pure phenomenological models, rather than models linked to the physics of accretion. In this paper, a detailed spectral study of the X-ray emission recorded from the high-mass X-ray binary pulsars Cen X-3, 4U 0115+63, and Her X-1 is carried out by using BeppoSAX and joined Suzaku+NuStar data, together with an advanced version of the compmag model. The latter provides a physical description of the high energy emission from accreting pulsars, including the thermal and bulk Comptonization of cyclotron and bremsstrahlung seed photons along the neutron star accretion column. The compmag model is based on an iterative method for solving second-order partial differential equations, whose convergence algorithm has been impr...

  3. Low-angle polarized neutron and X-ray scattering from magnetic nanolayers and nanostructures

    CERN Document Server

    Paul, Amitesh

    2017-01-01

    This research monograph presents the latest results related to the characterization of low dimensional systems. Low-angle polarized neutron scattering and X-ray scattering at grazing incidence are used as the two main techniques to explore various physical phenomena of these systems. Special focus is put on systems like thin film transition metal and rare-earth layers, oxide heterostructures, hybrid systems, self-assembled nanostructures and self-diffusion.  Readers will gain in-depth knowledge about the usage of specular scattering and off-specular scattering techniques. Investigation of in-plane and out-of-plane structures and magnetism with vector magnetometric information is illustrated comprehensively. The book caters to a wide audience working in the field of nano-dimensional magnetic systems and the neutron and X-ray reflectometry community in particular.

  4. Development of Resonant Soft X-ray Scattering for Polymer Systems at Advanced Light Source

    Science.gov (United States)

    Wang, Cheng; Hexemer, Alexander; Nasiatka, James; Chan, Elaine; Padmore, Howard

    2010-03-01

    It is envisioned that many polymer applications will rely on the heterogeneous morphologies of polymer blends or block copolymers to yield specific functional properties, such as organic light-emitting diodes and photovoltaics. Over the past few years, it has been strongly demonstrated that scattering at soft x-ray energies near the carbon K-edge yields chemically specific and enhanced contrast, thereby enabling structural studies of heterogeneous polymer films with thicknesses of only tens of nanometers. Resonant soft x-ray scattering (RSoXS) will provide the capability for a high-resolution chemical probe with interfacial sensitivity. We will discuss here the development of a dedicated RSoXS setup at the ALS Beamline 11.0.1, which is an elliptically polarized undulator beamline that covers the energy range of 200-1300 eV. It can accommodate a large variety of thin film samples and scattering geometries, including transmission, specular and off-specular reflection, as well as grazing incidence geometries, that will enable users to study both laterally- and depth-resolved structures. The generality, strength, and ease of RSoXS will have significant and immediate impacts in many areas of polymer science and technology. This will be achieved through systematic, collaborative studies of materials with potentially high impact applications.

  5. Evolution of intermediate-mass X-ray binaries driven by magnetic braking of Ap/Bp stars: I. ultracompact X-ray binaries

    CERN Document Server

    Chen, Wen-Cong

    2016-01-01

    It is generally believed that Ultracompact X-ray binaries (UCXBs) evolved from binaries consisting of a neutron star accreting from a low-mass white dwarf or helium star where mass transfer is driven by gravitational radiation. However, the standard white-dwarf evolutionary channel cannot produce the relatively long-period ($40 - 60$\\,min) UCXBs with high time-averaged mass-transfer rate. In this work, we explore an alternative evolutionary route toward UCXBs where the companions evolve from intermediate-mass Ap/Bp stars with an anomalously strong magnetic field ($100 - 10000$\\,G). Including the magnetic braking caused by the coupling between the magnetic field and an irradiation-driven wind induced by the X-ray flux from the accreting component, we show that intermediate-mass X-ray binaries (IMXBs) can evolve into UCXBs. Using the \\emph{MESA} code, we have calculated evolutionary sequences for a large number of IMXBs. The simulated results indicate that, for a small wind-driving efficiency $f=10^{-5}$, the a...

  6. The Relation Between Magnetic Fields and X-ray Emission for Solar Microflares and Active Regions

    Science.gov (United States)

    Kirichenko, A. S.; Bogachev, S. A.

    2017-09-01

    We present the result of a comparison between magnetic field parameters and the intensity of X-ray emission for solar microflares with Geosynchronous Operational Environmental Satellites (GOES) classes from A0.02 to B5.1. For our study, we used the monochromatic MgXII Imaging Spectroheliometer (MISH), the Full-disk EUV Telescope (FET), and the Solar PHotometer in X-rays (SphinX) instruments onboard the Complex Orbital Observations Near-Earth of Activity of the Sun-Photon CORONAS- Photon spacecraft because of their high sensitivity in soft X-rays. The peak flare flux (PFF) for solar microflares was found to depend on the strength of the magnetic field and on the total unsigned magnetic flux as a power-law function. In the spectral range 2.8 - 36.6 Å, which shows very little increase related to microflares, the power-law index of the relation between the X-ray flux and magnetic flux for active regions is 1.48 ±0.86, which is close to the value obtained previously by Pevtsov et al. ( Astrophys. J. 598, 1387, 2003) for different types of solar and stellar objects. In the spectral range 1 - 8 Å, the power-law indices for PFF(B) and PFF(Φ) for microflares are 3.87 ±2.16 and 3 ±1.6, respectively. We also make suggestions on the heating mechanisms in active regions and microflares under the assumption of loops with constant pressure and heating using the Rosner-Tucker-Vaiana scaling laws.

  7. Magnetic dichroism in angular resolved hard X-ray photoelectron spectroscopy from buried magnetic layers

    Energy Technology Data Exchange (ETDEWEB)

    ViolBarbosa, Carlos E.; Ouardi, Siham [Max Planck Institute for Chemical Physics of Solids, Nöthnitzer Str. 40, 01187 Dresden (Germany); Fecher, Gerhard H., E-mail: fecher@cpfs.mpg.de [Max Planck Institute for Chemical Physics of Solids, Nöthnitzer Str. 40, 01187 Dresden (Germany); Ebke, Daniel; Felser, Claudia [Max Planck Institute for Chemical Physics of Solids, Nöthnitzer Str. 40, 01187 Dresden (Germany)

    2013-08-15

    Highlights: ► We show the feasibility of angular resolved MCD in photospectroscopy. ► Wide-acceptance lens system allows a fixed incident light angle in the experiment. ► Bulk-sensitive HAXPES-MCDAD was used to study buried layers. ► Performance tools as Scalasca and Paraver are used to debug the applications. -- Abstract: This work reports on the measurement of magnetic dichroism in angular-resolved photoelectron spectroscopy from in-plane magnetized buried thin films. The high bulk sensitivity of hard X-ray photoelectron spectroscopy (HAXPES) in combination with circularly polarized radiation enables the investigation of the magnetic properties of buried layers. Angular distributions of high kinetic energy (7–8 keV) photoelectrons in a range of about 60° were recorded in parallel to the energy distribution. Depending on purpose, energy and angular resolutions of 150–250 meV and 0.17–2° can be accomplished simultaneously in such experiments. Experiments were performed on exchange-biased magnetic layers covered by thin oxide films. More specifically, the angular distribution of photoelectrons from the ferromagnetic layer Co{sub 2}FeAl layer grown on MnIr exchange-biasing layer was investigated where the magnetic structure is buried beneath a MgO layer. Pronounced magnetic dichroism is found in the Co and Fe 2p states for all angles of emission. A slightly increased magnetic dichroism was observed for normal emission in agreement with theoretical considerations.

  8. Relationship Between Solar Coronal X-Ray Brightness and Active Region Magnetic Fields: A Study Using High Resolution Observations

    CERN Document Server

    Hazra, Soumitra; Ravindra, B

    2014-01-01

    By utilizing high resolution observations of nearly co-temporal and co-spatial SOT spectropolarimeter and XRT coronal X-ray data onboard Hinode, we revisit the contentious issue of the relationship between global magnetic quantities and coronal X-ray intensity. Co-aligned vector magnetogram and X-ray data are used for this study. We find that there is no pixel-to-pixel correlation between the observed loop brightness and magnetic quantities. However, the X-ray brightness is well correlated with the integrated magnetic quantities such as total unsigned magnetic flux, total unsigned vertical current, area integrated square of the vertical magnetic field and horizontal magnetic fields. Comparing all these quantities we find that the total magnetic flux correlates well with the observed integrated X-ray brightness, though there is some differences in the strength of the correlation when we use the X-ray data from different filters. While we get a good correlation between X-ray brightness and total unsigned vertic...

  9. Design of Magnetic Shielding and Field Coils for a TES X-Ray Microcalorimeter Test Platform

    Science.gov (United States)

    Miniussi, Antoine R.; Adams, Joseph S.; Bandler, Simon R.; Chervenak, James A.; Datesman, Aaron M.; Doriese, William B.; Eckart, Megan E.; Finkbeiner, Fred M.; Kelley, Richard L.; Kilbourne, Caroline A.; hide

    2017-01-01

    The performance of Transition-Edge Sensors (TES) and their SQUID multiplexed read-outs are very sensitive to the ambient magnetic field from Earth and fluctuations that can arise due to fluctuating magnetic fields outside of the focal plane assembly from the Adiabatic Demagnetization Refrigerator (ADR).Thus, the experimental platform we are building to test the FPA of the X-ray Integral Field Unit (X-IFU) of the Athena mission needs to include a series of shields and a coil in order to meet the following requirement of magnetic field density and uniformity.

  10. A 1-D Study of the Ignition Space for Magnetic Indirect (X-ray) Drive Targets

    Energy Technology Data Exchange (ETDEWEB)

    Cobble, James Allen [Los Alamos National Lab. (LANL), Los Alamos, NM (United States); Sinars, Daniel Brian [Sandia National Lab. (SNL-NM), Albuquerque, NM (United States)

    2016-06-02

    The ICF program today is investigating three approaches to achieving multi-MJ fusion yields and ignition: (1) laser indirect (x-ray) drive on the National Ignition Facility (NIF), (2) laser direct drive (primarily on the Omega laser facility at the University of Rochester), and (3) magnetic direct drive on the Z pulsed power facility. In this white paper we briefly consider a fourth approach, magnetic indirect drive, in which pulsedpower- driven x-ray sources are used in place of laser driven sources. We first look at some of the x-ray sources studied on Z prior to 2007 before the pulsed power ICF program shifted to magnetic direct drive. We then show results from a series of 1D Helios calculations of double-shell capsules that suggest that these sources, scaled to higher temperatures, could be a promising path to achieving multi-MJ fusion yields and ignition. We advocate here that more detailed design calculations with widely accepted 2D/3D ICF codes should be conducted for a better assessment of the prospects.

  11. X-rays from Magnetically Confined Wind Shocks: Effect of Cooling-Regulated Shock Retreat

    CERN Document Server

    ud-Doula, Asif; Townsend, Richard; Petit, Veronique; Cohen, David

    2014-01-01

    We use 2D MHD simulations to examine the effects of radiative cooling and inverse Compton (IC) cooling on X-ray emission from magnetically confined wind shocks (MCWS) in magnetic massive stars with radiatively driven stellar winds. For the standard dependence of mass loss rate on luminosity $\\Mdot \\sim L^{1.7} $, the scaling of IC cooling with $L$ and radiative cooling with $\\Mdot$ means that IC cooling become formally more important for lower luminosity stars. However, because the sense of the trends is similar, we find the overall effect of including IC cooling is quite modest. More significantly, for stars with high enough mass loss to keep the shocks radiative, the MHD simulations indicate a linear scaling of X-ray luminosity with mass loss rate; but for lower luminosity stars with weak winds, X-ray emission is reduced and softened by a {\\em shock retreat} resulting from the larger post-shock cooling length, which within the fixed length of a closed magnetic loop forces the shock back to lower pre-shock w...

  12. Resonant K-alpha spectroscopy of a hot dense plasma created by the LCLS x-ray free electron laser

    Science.gov (United States)

    Cho, Byoung-Ick; Engelhorn, K.; Falcone, R. W.; Heimann, P. A.; Vinko, S. M.; Ciricosta, O.; Higginbotham, A.; Murphy, C.; Wark, J. S.; Chung, H.-K.; Brown, C. R. D.; Burian, T.; Vysin, L.; Juha, L.; Lee, H. J.; Messersmidt, M.; Schlotter, W.; Turner, J.; Nagler, B.; Ping, Y.; Lee, R. W.; Toleikis, S.; Zastrau, U.

    2011-10-01

    We present one of the first experimental studies of the interaction of high intensity x-ray free electron laser radiation with solid density matter. In the experiment performed at the LCLS, an intense 80 fs x-ray pulse at 1017 Wcm-2 with photon energies of 1480 ~ 1560 eV is focused on a thin Al foil and K-alpha emission spectra are observed. Although x-ray photon energy is lower than the absorption edge, because of its high intensity the sample is surprisingly heated up to 100 ~200 eV in the pulse duration and a hot dense plasma is created. Observed x-ray spectra indicate this dense plasma resonantly interacts with the x-ray photons. The emission spectra are also simulated using the collisional-radiative code, SCFLY which provides information about the electron temperature and density, the charge state distribution and opacity. The comparison of experiment and simulation provides a detailed description of a dense plasma resonantly interacting with an intense x-ray pulse.

  13. Onset of the Magnetic Explosion in Solar Polar Coronal X-Ray Jets

    Science.gov (United States)

    Moore, Ronald L.; Sterling, Alphonse C.; Panesar, Navdeep

    2017-08-01

    We examine the onset of the driving magnetic explosion in 15 random polar coronal X-ray jets. Each eruption is observed in a coronal X-ray movie from Hinode and in a coronal EUV movie from Solar Dynamics Observatory. Contrary to the Sterling et al (2015, Nature, 523, 437) scenario for minifilament eruptions that drive polar coronal jets, these observations indicate: (1) in most polar coronal jets (a) the runaway internal tether-cutting reconnection under the erupting minifilament flux rope starts after the spire-producing breakout reconnection starts, not before it, and (b) aleady at eruption onset, there is a current sheet between the explosive closed magnetic field and ambient open field; and (2) the minifilament-eruption magnetic explosion often starts with the breakout reconnection of the outside of the magnetic arcade that carries the minifilament in its core. On the other hand, the diversity of the observed sequences of occurrence of events in the jet eruptions gives further credence to the Sterlling et al (2015, Nature, 523, 437) idea that the magnetic explosions that make a polar X-ray jet work the same way as the much larger magnetic explosions that make and flare and CME. We point out that this idea, and recent observations indicating that magnetic flux cancelation is the fundamental process that builds the field in and around pre-jet minifilaments and triggers the jet-driving magnetic explosion, together imply that usually flux cancelation inside the arcade that explodes in a flare/CME eruption is the fundamental process that builds the explosive field and triggers the explosion.This work was funded by the Heliophysics Division of NASA's Science Mission Directorate through its Living With a Star Targeted Research and Technology Program, its Heliophsyics Guest Investigators Program, and the Hinode Project.

  14. Microwave soft x-ray microscopy for nanoscale magnetization dynamics in the 5–10 GHz frequency range

    Energy Technology Data Exchange (ETDEWEB)

    Bonetti, Stefano, E-mail: bonetti@slac.stanford.edu; Chen, Zhao [Department of Physics, Stanford University, Stanford, California 94305 (United States); Stanford Institute for Materials and Energy Sciences, SLAC National Accelerator Laboratory, 2575 Sand Hill Road, Menlo Park, California 94025 (United States); Kukreja, Roopali [Stanford Institute for Materials and Energy Sciences, SLAC National Accelerator Laboratory, 2575 Sand Hill Road, Menlo Park, California 94025 (United States); Department of Materials Science and Engineering, Stanford University, Stanford, California 94305 (United States); Spoddig, Detlef; Schöppner, Christian; Meckenstock, Ralf [Institut für Experimentalphysik, Universität Duisburg-Essen, Duisburg (Germany); Ollefs, Katharina [Institut für Experimentalphysik, Universität Duisburg-Essen, Duisburg (Germany); European Synchrotron Radiation Facility, 38043 Grenoble Cedex (France); Ney, Andreas [Institut für Experimentalphysik, Universität Duisburg-Essen, Duisburg (Germany); Solid State Physics Division, Johannes Kepler University, 4040 Linz (Austria); Pinto, Jude; Houanche, Richard; Frisch, Josef [Linear Coherent Light Source, SLAC National Accelerator Laboratory, Menlo Park, California 94025 (United States); Stöhr, Joachim; Dürr, Hermann A. [Stanford Institute for Materials and Energy Sciences, SLAC National Accelerator Laboratory, 2575 Sand Hill Road, Menlo Park, California 94025 (United States); Ohldag, Hendrik [Stanford Synchrotron Radiation Laboratory, SLAC National Accelerator Laboratory, Menlo Park, California 94025 (United States)

    2015-09-15

    We present a scanning transmission x-ray microscopy setup combined with a novel microwave synchronization scheme for studying high frequency magnetization dynamics at synchrotron light sources. The sensitivity necessary to detect small changes in the magnetization on short time scales and nanometer spatial dimensions is achieved by combining the excitation mechanism with single photon counting electronics that is locked to the synchrotron operation frequency. Our instrument is capable of creating direct images of dynamical phenomena in the 5-10 GHz range, with high spatial resolution. When used together with circularly polarized x-rays, the above capabilities can be combined to study magnetic phenomena at microwave frequencies, such as ferromagnetic resonance (FMR) and spin waves. We demonstrate the capabilities of our technique by presenting phase resolved images of a ∼6 GHz nanoscale spin wave generated by a spin torque oscillator, as well as the uniform ferromagnetic precession with ∼0.1° amplitude at ∼9 GHz in a micrometer-sized cobalt strip.

  15. Sub-100 nanometer lensless probing of Co/Pd magnetic nanodomains using a table-top femtosecond soft X-ray harmonic source

    Science.gov (United States)

    Ge, X.; Ducousso, M.; Boutu, W.; Tudu, B.; Barbrel, B.; Gauthier, D.; Borta, A.; Gonzalez, A.-I.; Wang, F.; Iwan, B.; Billon, M.; Perdrix, M.; Guillaumet, D.; Lepetit, F.; Vodungbo, B.; Gautier, J.; Hawaldar, R.; Tortarolo, M.; Delaunay, R.; Zeitoun, P.; Lüning, J.; Merdji, H.

    2013-10-01

    We present recent developments of our table-top femtosecond high flux harmonic beamline towards single-shot probing of magnetic nanostructures. High harmonic generation (HHG) optimization in a single and two-color infrared laser pulse mode was investigated at high laser energy. Up to 109 photons per harmonic are generated between 40 and 80 eV in a single femtosecond laser shot. These soft X-ray harmonic photons are employed to characterize at the nanoscale the magnetic network of Co/Pd multilayer samples using resonant small-angle X-ray scattering. Selecting harmonics in the vicinity of magnetically dichroic absorption resonances of cobalt and palladium (Co M2,3 at 60 eV and Pd N2,3 at 51 eV) gives access to the magnetic nanodomain spatial structure. The magnetic scattering efficiency at the Pd edge is found to be comparable to that at the Co edge. This indicates that the Pd layers exhibit a significant induced magnetic moment. Magnetic sample optimization is then performed by characterizing its scattering efficiency as a function of layer composition and number of repetitions. We finally measure the spatial organization of magnetic nanodomains with a sub-100 nm spatial resolution from a single femtosecond X-ray pulse.

  16. Resonant x-ray scattering in perovskite manganite superlattice. Observation of 'orbital superlattice'

    CERN Document Server

    Kiyama, T; Ohsumi, H; Murakami, Y; Wakabayashi, Y; Izumi, M; Kawasaki, M; Tokura, Y

    2003-01-01

    We report the results of resonant X-ray scattering (RXS) measurement of superlattices which consist of La sub 0 sub . sub 4 sub 5 Sr sub 0 sub . sub 5 sub 5 MnO sub 3 and La sub 0 sub . sub 6 sub 0 Sr sub 0 sub . sub 4 sub 0 MnO sub 3 multilayers. An interference technique made it possible to observe RXS reflections from ferro-type orbital ordering in the superlattices. RXS can reveal the local circumstances around specific atoms in materials regulated atomically. In this experiment, we observed that the superlattice is actually composed of two kinds of layers with different lattice distortion states, presenting 'orbital superlattices', in which layers with different orbital states are stacked alternately in an atomic scale. (author)

  17. Some notes on data analysis for nuclear resonant inelastic x-ray scattering

    Science.gov (United States)

    Hu, Michael Y.

    2016-12-01

    Nuclear Resonant Inelastic X-ray Scattering (NRIXS) is a spectroscopy method to study atomic vibrations and dynamics, currently done with synchrotron radiation at a few high energy third generation facilities. It finds a wide range of applications in condensed matter physics, materials science, chemistry, biophysics, geosciences, and high-pressure researches. Many atomic dynamics and lattice thermodynamics information can be derived from NRIXS measurements. Phonon Density of States (DOS) characterizes lattice dynamics of a material and can be derived under the quasi-harmonic approximation. Combined with modeling and simulations, results from NRIXS can provide unique and clarifying insights into many fields of research. As for a spectroscopic technique, in order to be able to provide reliable information, close attention should be paid to many issues during experiments and data analysis afterwards. Here we discuss several issues relevant to its data analysis, namely, those of multiple sites, background treatments, and error estimates for some derived quantities.

  18. Some notes on data analysis for nuclear resonant inelastic x-ray scattering

    Energy Technology Data Exchange (ETDEWEB)

    Hu, Michael Y., E-mail: myhu@aps.anl.gov [Argonne National Laboratory (United States)

    2016-12-15

    Nuclear Resonant Inelastic X-ray Scattering (NRIXS) is a spectroscopy method to study atomic vibrations and dynamics, currently done with synchrotron radiation at a few high energy third generation facilities. It finds a wide range of applications in condensed matter physics, materials science, chemistry, biophysics, geosciences, and high-pressure researches. Many atomic dynamics and lattice thermodynamics information can be derived from NRIXS measurements. Phonon Density of States (DOS) characterizes lattice dynamics of a material and can be derived under the quasi-harmonic approximation. Combined with modeling and simulations, results from NRIXS can provide unique and clarifying insights into many fields of research. As for a spectroscopic technique, in order to be able to provide reliable information, close attention should be paid to many issues during experiments and data analysis afterwards. Here we discuss several issues relevant to its data analysis, namely, those of multiple sites, background treatments, and error estimates for some derived quantities.

  19. X-Ray Magnetic Circular Dichroism Measurement of Fe-Co Alloy Films Prepared by Electrodeposition

    Institute of Scientific and Technical Information of China (English)

    LI Zong-Mu; XU Fa-Qiang; WANG Li-Wu; WANG Jie; ZHU Jun-Fa; ZHANG Wen-Hua

    2007-01-01

    The macro- and micro-magnetic properties of Fe-Co alloy films eletrodeposited on GaAs(100) are studied by synchrotron radiation x-ray magnetic circular dichroism (XMCD) in combination with the magneto-optical Kerr effect (MOKE) measurements and magnetic force microscopy (MFM). The orbital and spin magnetic moments of each element in the Fe-Co alloy are determined by the sum rules of XMCD. Element-specific hysteresis loops (ESHL) are obtained by recording the La MCD signals as a function of applied magnetic field. MOKE results reveal that the amorphous films are magnetically isotropic in the surface plane. The MFM image shows that the dimension of the magnetic domains is about 1-2 μm, which is much larger than that of the grains, indicating that there are intergranular correlations among these grains. Both ESHL and MOKE hysteresis loops indicate the strong ferromagnetic coupling of Fe and Co in the alloy films.

  20. Ultrasensitive Scanning Transmission X-ray Microscopy: Pushing the Limits of Time Resolution and Magnetic Sensitivity

    Science.gov (United States)

    Ohldag, Hendrik

    Understanding magnetic properties at ultrafast timescales is crucial for the development of new magnetic devices. Samples of interest are often thin film magnetic multilayers with thicknesses in the range of a few atomic layers. This fact alone presents a sensitivity challenge in STXM microscopy, which is more suited toward studying thicker samples. In addition the relevant time scale is of the order of 10 ps, which is well below the typical x-ray pulse length of 50 - 100 ps. The SSRL STXM is equipped with a single photon counting electronics that effectively allows using a double lock-in detection at 476MHz (the x-ray pulse frequency) and 1.28MHz (the synchrotron revelation frequency) to provide the required sensitivity. In the first year of operation the excellent spatial resolution, temporal stability and sensitivity of the detection electronics of this microscope has enabled researchers to acquire time resolved images of standing as well as traveling spin waves in a spin torque oscillator in real space as well as detect the real time spin accumulation in non magnetic Copper once a spin polarized current is injected into this material. The total magnetic moment is comparable to that of a single nanocube of magnetic Fe buried under a micron of non-magnetic material.

  1. The structural and magnetic properties of Fe/native-oxide systems resolved by x-ray scattering and spectroscopy methods

    Energy Technology Data Exchange (ETDEWEB)

    Couet, Sebastien

    2008-12-15

    Since the discovery of the giant magnetoresistance (GMR) effect in metallic magnetic multilayers and its industrial application in magnetic read heads, the data storage density and reading speed of hard disks steadily increased. But now the point is reached where conventional conductive multilayer structures suffer from parasitic eddy currents which decrease the signal to noise ratio of the system. To tackle this problem, new classes of materials have to be studied. One approach is to introduce ultra thin oxide layers in a metallic iron structure to reduce the conductivity while keeping a high net magnetization. This can be achieved by alternating metal deposition and controlled oxidation to produce metal/metal-oxide multilayers. However, the magnetic structure that forms in such multilayer is still rather unexplored. The aim of this work was to achieve a better understanding of the magnetic structure that forms in such iron/native-oxide multilayers. For that purpose, X-ray and neutron scattering experiments were carried out to determine the magnetic structure and its evolution in ex-situ and in-situ experiments, respectively. It was found that a non-collinear magnetic coupling appears between the metal layers, which is mediated by the antiferromagnetically ordered oxide layer in between. The use of isotope sensitive scattering techniques (namely nuclear resonant scattering and neutron reflectometry) allowed to resolve the magnetic depth profile of the system, showing that the buried oxide carries a net magnetic moment. The chemical and magnetic structure of the buried oxide was studied by in-situ X-ray absorption spectroscopy and nuclear resonant scattering. After oxidation, the layer exhibits a mixture of different oxide phases and incorporates 10 to 15% of Fe with metallic character. Upon deposition of only one atomic layer of metallic Fe, the layer reduces to a single phase FeO-like oxide. This structural change does not lead to a magnetically ordered oxide

  2. Thermal and magnetic anomalies of α-iron: an exploration by extended x-ray absorption fine structure spectroscopy and synchrotron x-ray diffraction

    Science.gov (United States)

    Boccato, Silvia; Sanson, Andrea; Kantor, Innokenty; Mathon, Olivier; Dyadkin, Vadim; Chernyshov, Dmitry; Carnera, Alberto; Pascarelli, Sakura

    2016-09-01

    The local structure and dynamics of α-iron have been investigated by extended x-ray absorption fine structure (EXAFS) spectroscopy and x-ray diffraction (XRD) in order to shed light on some thermal and magnetic anomalies observed in the last decades. The quantitative EXAFS analysis of the first two coordination shells reveals a peculiar local vibrational dynamics of α-iron: the second neighbor distance exhibits anharmonicity and vibrational anisotropy larger than the first neighbor distance. We search for possible distortions of the bcc structure to justify the unexplained magnetostriction anomalies of α-iron and provide a value for the maximum dislocation of the central Fe atom. No thermal anomalies have been detected from the current XRD data. On the contrary, an intriguing thermal anomaly at about 150 K, ascribed to a stiffening of the Fe-Fe bonds, was found by EXAFS.

  3. 钼靶X线、超声及MRI在乳腺癌诊断中的协同应用%Collaborative Application of Molybdenum Target X-ray, Ultrasonography, and Magnetic Resonance Imaging in the Diagnosis of Breast Cancer

    Institute of Scientific and Technical Information of China (English)

    李旭敏; 薛红芳; 李卉

    2016-01-01

    目的:探讨钼靶X线、超声和动态增强MRI在乳腺癌诊断中的协同应用价值。方法选择2012年6月~2014年12月于邢台市中医院就诊的112例乳腺癌疑似病例,分别给予钼靶X线、超声和动态增强MRI检查,将检查结果与术后病理诊断结果进行比较,评价各方法以及3种方法联用的诊断价值。结果 MRI的诊断灵敏度、特异度、准确度明显高于超声、钼靶X线(P0.05)。钼靶X线的钙化显示率明显高于超声和MRI诊断(P0.05). The calcification display rate of molybdenum target X-ray was significantly higher than that of the ultrasound and MRI (P<0.05). Conclusion The sensitivity, specificity and accuracy of MRI in the diagnosis of breast cancer were higher than those of molybdenum target X-ray and ultrasonography. Yet these three diagnostic methods had their own insufficiencies. Therefore, a reasonably collaborative application of the three methods could improve the accuracy of diagnosis of breast cancer.

  4. Measurement of vertebral bone marrow lipid profile at 1.5-T proton magnetic resonance spectroscopy and bone mineral density at dual-energy X-ray absorptiometry: correlation in a swine model

    Energy Technology Data Exchange (ETDEWEB)

    Di Leo, Giovanni; Fina, Laura [IRCCS Policlinico San Donato, Unita di Radiologia, San Donato Milanese (Italy); Bandirali, Michele; Messina, Carmelo [Universita degli Studi di Milano, Scuola di Specializzazione in Radiodiagnostica, Milan (Italy); Sardanelli, Francesco [IRCCS Policlinico San Donato, Unita di Radiologia, San Donato Milanese (Italy); Universita degli Studi di Milano, Dipartimento di Scienze Biomediche per la Salute, San Donato Milanese (Italy)

    2014-08-15

    Bone marrow is mainly composed of red (hematopoietic) and yellow (fatty) components. Soon after the birth there is a physiological conversion of the bone marrow from red to yellow, so that the percentage of hematopoietic cells and adipocytes changes with aging. Although bone marrow adipogenesis is a physiologic process involving all mammals, recent studies showed an accelerated marrow adipogenesis associated with several chronic conditions, including osteoporosis [4] and diabetes mellitus. Moreover, this increased marrow fat is accompanied by a decrease in bone density. Marrow fat is therefore increasingly believed to influence the bone microenvironment. Diagnostic tools for quantitative measurement of bone marrow fat and bone mineral density (BMD) include proton magnetic resonance spectroscopy (MRS) and dual-energy Xray absorptiometry (DXA), respectively. Using MRS, an inverse relationship between vertebral bone marrow fat content and lumbar BMD has been demonstrated in patients affected with osteoporosis or with diabetes mellitus. In most studies, a quite standard MRS sequence has been used, with short echo times (TE) for the measurement of the bulk methylene. In this study we sought to optimize the MRS sequence in order to try to measure other fat components of the vertebral bone marrow at 1.5 T. For this purpose, we used an animal model that allowed long acquisition times and repeated measures. Moreover, we aimed at estimating in this model the relationship between vertebral bone marrow fat content at proton MRS and BMD at DXA.

  5. First-principles analysis of X-ray magnetic circular dichroism for transition metal complex oxides

    Science.gov (United States)

    Ikeno, Hidekazu

    2016-10-01

    X-ray magnetic circular dichroism (XMCD) is widely used for the characterization of magnetism of materials. However, information from XMCD related to the atomic, electronic, and magnetic structures is not fully utilized due to the lack of reliable theoretical tools for spectral analysis. In this work, the first-principles configuration interaction (CI) calculations for X-ray absorption spectra developed by the author were extended for the calculation of XMCD, where the Zeeman energy was taken into the Hamiltonian of the CI to mimic magnetic polarization in the solid state. This technique was applied to interpret the L2,3 XMCD from 3d transition metal complex oxides, such as NiFe2O4 and FeTiO3. The experimental XMCD spectra were quantitatively reproduced using this method. The oxidation states as well as the magnetic ordering between transition metal ions on crystallographically different sites in NiFe2O4 can be unambiguously determined. A first-principles analysis of XMCD in FeTiO3 revealed the presence of Fe3+ and Ti3+ ions, which indicates that the charge transfer from Fe to Ti ions occurs. The origin of magnetic polarization of Ti ions in FeTiO3 was also discussed.

  6. First-principles analysis of X-ray magnetic circular dichroism for transition metal complex oxides

    Energy Technology Data Exchange (ETDEWEB)

    Ikeno, Hidekazu, E-mail: h-ikeno@21c.osakafu-u.ac.jp [Nanoscience and Nanotechnology Research Center, Research Organization for the 21st Century, Osaka Prefecture University, 1-2 Gakuen-cho, Naka-ku, Sakai, Osaka 599-8570 (Japan)

    2016-10-14

    X-ray magnetic circular dichroism (XMCD) is widely used for the characterization of magnetism of materials. However, information from XMCD related to the atomic, electronic, and magnetic structures is not fully utilized due to the lack of reliable theoretical tools for spectral analysis. In this work, the first-principles configuration interaction (CI) calculations for X-ray absorption spectra developed by the author were extended for the calculation of XMCD, where the Zeeman energy was taken into the Hamiltonian of the CI to mimic magnetic polarization in the solid state. This technique was applied to interpret the L{sub 2,3} XMCD from 3d transition metal complex oxides, such as NiFe{sub 2}O{sub 4} and FeTiO{sub 3}. The experimental XMCD spectra were quantitatively reproduced using this method. The oxidation states as well as the magnetic ordering between transition metal ions on crystallographically different sites in NiFe{sub 2}O{sub 4} can be unambiguously determined. A first-principles analysis of XMCD in FeTiO{sub 3} revealed the presence of Fe{sup 3+} and Ti{sup 3+} ions, which indicates that the charge transfer from Fe to Ti ions occurs. The origin of magnetic polarization of Ti ions in FeTiO{sub 3} was also discussed.

  7. Phase quantification in nanobainite via magnetic measurements and X-ray diffraction

    Energy Technology Data Exchange (ETDEWEB)

    Solano-Alvarez, W., E-mail: ws298@cam.ac.uk [Department of Materials Science and Metallurgy, University of Cambridge (United Kingdom); Abreu, H.F.G. [Departamento de Engenharia Metalúrgica e de Materiais, Universidade Federal do Ceará, Fortaleza (Brazil); Silva, M.R. da [Instituto de Física e Química, Universidade Federal de Itajubá, Itajubá, Minas Gerais (Brazil); Peet, M.J. [Department of Materials Science and Metallurgy, University of Cambridge (United Kingdom)

    2015-03-15

    Accurate phase quantification of nanostructured bainitic steel is of importance because of the nature of its percolating structure that controls many of its mechanical properties. X-ray diffraction is the technique of choice for such analysis, but magnetic methods can be more rapid and less sensitive to defect structures. In this study, the phase volume fractions measured using both of these techniques for the specific mixtures associated with nanostructured bainite have been compared and contrasted. An expression which relates the volume fraction and the saturation magnetization is obtained and its form is found to be consistent with previous work done on duplex stainless steels and TRIP steels. The fitting constants used in many of such analyses vary significantly so an attempt is made to rationalize the differences by considering the factors that determine the intrinsic saturation magnetization of ferrite. - Author-Highlights: • Magnetic phase quantification of nanobainite is presented for the first time. • Results are compared with x-ray diffraction. • Expression obtained that relates ferrite fraction and saturation magnetization. • Equation derived to calculate intrinsic saturation magnetization of ferrites. • These values agree with experimental data of the literature.

  8. The space density and X-ray luminosity function of non-magnetic cataclysmic variables

    Science.gov (United States)

    Pretorius, Magaretha L.; Knigge, Christian

    2012-01-01

    We combine two complete, X-ray flux-limited surveys, the ROSAT Bright Survey (RBS) and the ROSAT North Ecliptic Pole (NEP) survey, to measure the space density (ρ) and X-ray luminosity function (Φ) of non-magnetic cataclysmic variables (CVs). The combined survey has a flux limit of FX≳ 1.1 × 10-12 erg cm-2 s-1 over most of its solid angle of just over ?, but is as deep as ≃10-14 erg cm-2 s-1 over a small area. The CV sample that we construct from these two surveys contains 20 non-magnetic systems. We carefully include all sources of statistical error in calculating ρ and Φ by using Monte Carlo simulations; the most important uncertainty proves to be the often large errors in distances estimates. If we assume that the 20 CVs in the combined RBS and NEP survey sample are representative of the intrinsic population, the space density of non-magnetic CVs is ?. We discuss the difficulty in measuring Φ in some detail - in order to account for biases in the measurement, we have to adopt a functional form for Φ. Assuming that the X-ray luminosity function of non-magnetic CVs is a truncated power law, we constrain the power-law index to -0.80 ± 0.05. It seems likely that the two surveys have failed to detect a large, faint population of short-period CVs, and that the true space density may well be a factor of 2 or 3 larger than what we have measured; this is possible, even if we only allow for undetected CVs to have X-ray luminosities in the narrow range 28.7 log(LX/erg s-1) < 29.7. However, ρ as high as 2 × 10-4 pc-3 would require that the majority of CVs has X-ray luminosities below LX= 4 × 1028 erg s-1 in the 0.5-2.0 keV band.

  9. X-ray absorption and magnetic circular dichroism studies of Co2FeAl in magnetic tunnel junctions

    Energy Technology Data Exchange (ETDEWEB)

    Ebke, D.; Kugler, Z.; Thomas, P.; Schebaum, O.; Schafers, M.; Nissen, D.; Schmalhorst, J.; Hutten, A.; Arenholz, E.; Thomas, A.

    2010-01-11

    The bulk magnetic moment and the element specific magnetic moment of Co{sub 2}FeAl thin films were examined as a function of annealing temperature by alternating gradient magnetometer (AGM) and X-ray absorption spectroscopy (XAS)/X-ray magnetic circular dichroism (XMCD), respectively. A high magnetic moment can be achieved for all annealing temperatures and the predicted bulk and interface magnetic moment of about 5 {tilde A}{sub B} are reached via heating. We will also present tunnel magnetoresistance (TMR) values of up to 153% at room temperature and 260% at 13 K for MgO based magnetic tunnel junctions (MTJs) with Co{sub 2}FeAl and Co-Fe electrodes.

  10. Studies of SmCo5/Fe nanocomposite magnetic bilayers with magnetic soft x-ray transmission microscopy

    Energy Technology Data Exchange (ETDEWEB)

    Shahzad, F.; Siddiqi, S. A.; Im, M.-Y.; Avallone, A.; Fischer, P.; Hussain, Z.; Siddiqi, I.; Hellman, F.; Zhao, J.

    2009-12-04

    A hard/soft SmCo{sub 5}/Fe nanocomposite magnetic bilayer system has been fabricated on X-ray transparent 100-200 nm thin Si{sub 3}N{sub 4} membranes by magnetron sputtering. The microscopic magnetic domain pattern and its behavior during magnetization reversal in the hard and soft magnetic phases have been individually studied by element specific magnetic soft x-ray microscopy at a spatial resolution of better than 25nm. We observe that the domain patterns for soft and hard phases switch coherently throughout the full hysteresis cycle upon applying external magnetic fields. We derived local M(H) curves from the images for Fe and SmCo5 separately and found switching for both hard and soft phases same.

  11. Evolution of Intermediate-mass X-Ray Binaries Driven by the Magnetic Braking of AP/BP Stars. I. Ultracompact X-Ray Binaries

    Science.gov (United States)

    Chen, Wen-Cong; Podsiadlowski, Philipp

    2016-10-01

    It is generally believed that ultracompact X-ray binaries (UCXBs) evolved from binaries consisting of a neutron star accreting from a low-mass white dwarf (WD) or helium star where mass transfer is driven by gravitational radiation. However, the standard WD evolutionary channel cannot produce the relatively long-period (40-60 minutes) UCXBs with a high time-averaged mass-transfer rate. In this work, we explore an alternative evolutionary route toward UCXBs, where the companions evolve from intermediate-mass Ap/Bp stars with an anomalously strong magnetic field (100-10,000 G). Including the magnetic braking caused by the coupling between the magnetic field and an irradiation-driven wind induced by the X-ray flux from the accreting component, we show that intermediate-mass X-ray binaries (IMXBs) can evolve into UCXBs. Using the MESA code, we have calculated evolutionary sequences for a large number of IMXBs. The simulated results indicate that, for a small wind-driving efficiency f = 10-5, the anomalous magnetic braking can drive IMXBs to an ultra-short period of 11 minutes. Comparing our simulated results with the observed parameters of 15 identified UCXBs, the anomalous magnetic braking evolutionary channel can account for the formation of seven and eight sources with f = 10-3, and 10-5, respectively. In particular, a relatively large value of f can fit three of the long-period, persistent sources with a high mass-transfer rate. Though the proportion of Ap/Bp stars in intermediate-mass stars is only 5%, the lifetime of the UCXB phase is ≳2 Gyr, producing a relatively high number of observable systems, making this an alternative evolutionary channel for the formation of UCXBs.

  12. PREFACE: REXS 2013 - Workshop on Resonant Elastic X-ray Scattering in Condensed Matter

    Science.gov (United States)

    Beutier, G.; Mazzoli, C.; Yakhou, F.; Brown, S. D.; Bombardi, A.; Collins, S. P.

    2014-05-01

    The aim of this workshop was to bring together experts in experimental and theoretical aspects of resonant elastic x-ray scattering, along with researchers who are new to the field, to discuss important recent results and the fundamentals of the technique. The meeting was a great success, with the first day dedicated to students and new researchers in the field, who received introductory lectures and tutorials. All conference delegates were invited either to make an oral presentation or to present a poster, accompanied by a short talk. The first two papers selected for the REXS13 proceedings (Grenier & Joly and Helliwell) give a basic background to the theory of REXS and applications across a wide range of scientific areas. The remainder of the papers report on some of the latest scientific results obtained by applying the REXS technique to contemporary problems in condensed matter, materials and x-ray physics. It is hoped that these proceedings provide a snapshot of the current status of a vibrant and diverse scientific technique that will be of value not just to those who attended the workshop but also to any other reader with an interest in the subject. Local Scientific Committee REXS13 International Scientific Advisory Committee M Altarelli, European XFEL, Germany F de Bergevin, European Synchrotron Radiation Facility, France J Garcia-Ruiz, Universidad de Zaragoza, Spain A I Goldman, Iowa State University, USA M Goldmann, Institut Nanosciences, France T Schulli, European Synchrotron Radiation Facility, France C R Natoli, Laboratori Nazionali de Frascati, Italy G Materlik, Diamond Light Source, UK L Paolasini, European Synchrotron Radiation Facility, France U Staub, Paul Scherrer Institut, Switzerland K Finkelstein, Cornell University, USA Y Murakami, Photon Factory, Japan REXS13 Local Scientific Committee G Beutier, CNRS Grenoble, France C Mazzoli, Politecnico di Milano, Italy F Yakhou, European Synchrotron Radiation Facility, France S D Brown, XMaS UK CRG

  13. Interferometric phase detection at x-ray energies via Fano resonance control

    CERN Document Server

    Heeg, K P; Schumacher, D; Wille, H -C; Röhlsberger, R; Pfeifer, T; Evers, J

    2014-01-01

    Modern x-ray light sources promise access to structure and dynamics of matter in largely unexplored spectral regions. However, the desired information is encoded in the light intensity and phase, whereas detectors register only the intensity. This phase problem is ubiquitous in crystallography and imaging, and impedes the exploration of quantum effects at x-ray energies. Here, we demonstrate phase-sensitive measurements characterizing the quantum state of a nuclear two-level system at hard x-ray energies. The nuclei are initially prepared in a superposition state. Subsequently, the relative phase of this superposition is interferometrically reconstructed from the emitted x-rays. Our results form a first step towards x-ray quantum state tomography, and provide new avenues for structure determination and precision metrology via x-ray Fano interference.

  14. X-ray imaging of vortex cores in confined magnetic structures

    Energy Technology Data Exchange (ETDEWEB)

    Fischer, P; Im, M -Y; Kasai, S; Yamada, K; Ono, T; Thiaville, A

    2011-02-11

    Cores of magnetic vortices in micron-sized NiFe disk structures, with thicknesses between 150 and 50 nm, were imaged and analyzed by high-resolution magnetic soft x-ray microscopy. A decrease of the vortex-core radius was observed from approximately 38 to 18 nm with decreasing disk thickness. By comparing with full three-dimensional micromagnetic simulations showing the well-known barrel structure, we obtained excellent agreement, taking into account instrumental broadening and a small perpendicular anisotropy. The proven magnetic spatial resolution of better than 25 nm was sufficient to identify a negative dip close to the vortex core, originating from stray fields of the core. Magnetic vortex structures can serve as test objects for evaluating sensitivity and spatial resolution of advanced magnetic microscopy techniques.

  15. X-Ray Emission Spectrometer Design with Single-Shot Pump-Probe and Resonant Excitation Capabilities

    Energy Technology Data Exchange (ETDEWEB)

    Spoth, Katherine; /SUNY, Buffalo /SLAC

    2012-08-28

    Core-level spectroscopy in the soft X-ray regime is a powerful tool for the study of chemical bonding processes. The ultrafast, ultrabright X-ray pulses generated by the Linac Coherent Light Source (LCLS) allow these reactions to be studied in greater detail than ever before. In this study, we investigated a conceptual design of a spectrometer for the LCLS with imaging in the non-dispersive direction. This would allow single-shot collection of X-ray emission spectroscopy (XES) measurements with varying laser pump X-ray probe delay or a variation of incoming X-ray energy over the illuminated area of the sample. Ray-tracing simulations were used to demonstrate how the components of the spectrometer affect its performance, allowing a determination of the optimal final design. These simulations showed that the spectrometer's non-dispersive focusing is extremely sensitive to the size of the sample footprint; the spectrometer is not able to image a footprint width larger than one millimeter with the required resolution. This is compatible with a single shot scheme that maps out the laser pump X-ray probe delay in the non-dispersive direction as well as resonant XES applications at normal incidence. However, the current capabilities of the Soft X-Ray (SXR) beamline at the LCLS do not produce the required energy range in a small enough sample footprint, hindering the single shot resonant XES application at SXR for chemical dynamics studies at surfaces. If an upgraded or future beamline at LCLS is developed with lower monochromator energy dispersion the width can be made small enough at the required energy range to be imaged by this spectrometer design.

  16. Performance Verification of the Gravity and Extreme Magnetism Small Explorer GEMS X-Ray Polarimeter

    Science.gov (United States)

    Enoto, Teruaki; Black, J. Kevin; Kitaguchi, Takao; Hayato, Asami; Hill, Joanne E.; Jahoda, Keith; Tamagawa, Toru; Kanako, Kenta; Takeuchi, Yoko; Yoshikawa, Akifumi; Kenward, David

    2014-01-01

    olarimetry is a powerful tool for astrophysical observations that has yet to be exploited in the X-ray band. For satellite-borne and sounding rocket experiments, we have developed a photoelectric gas polarimeter to measure X-ray polarization in the 2-10 keV range utilizing a time projection chamber (TPC) and advanced micro-pattern gas electron multiplier (GEM) techniques. We carried out performance verification of a flight equivalent unit (1/4 model) which was planned to be launched on the NASA Gravity and Extreme Magnetism Small Explorer (GEMS) satellite. The test was performed at Brookhaven National Laboratory, National Synchrotron Light Source (NSLS) facility in April 2013. The polarimeter was irradiated with linearly-polarized monochromatic X-rays between 2.3 and 10.0 keV and scanned with a collimated beam at 5 different detector positions. After a systematic investigation of the detector response, a modulation factor greater than or equal to 35% above 4 keV was obtained with the expected polarization angle. At energies below 4 keV where the photoelectron track becomes short, diffusion in the region between the GEM and readout strips leaves an asymmetric photoelectron image. A correction method retrieves an expected modulation angle, and the expected modulation factor, approximately 20% at 2.7 keV. Folding the measured values of modulation through an instrument model gives sensitivity, parameterized by minimum detectable polarization (MDP), nearly identical to that assumed at the preliminary design review (PDR).

  17. Performance and Characterization of Magnetic Penetration Thermometer Devices for X-Ray Spectroscopy

    Science.gov (United States)

    Porst, J. -P.; Adams, J. S.; Bandler, S. R.; Balvin, M.; Busch, S. E.; Denis, K. L.; Kelly, D.; Nagler, P.; Sadleir, J. E.; Seidel, G. M.; Smith, S.; Stevenson, T. R.

    2012-01-01

    We are developing magnetic penetration thermometers (MPTs) for applications in X-ray astronomy. These non-dissipative devices consist of an X-ray absorber in good thermal contact to a superconducting thin film with a transition temperature around T=100mK. A microfabricated superconducting planar inductor underneath is used to store a persistent current and couple the superconductor's diamagnetic response to a readout SQUID. The strong temperature dependence of the diamagnetic response make these devices suitable for highly sensitive macroscopic thermometers that are capable of achieving very high energy resolution. We present results achieved with MPTs consisting of MoAu bilayer sensors attached to overhanging square 250 micron by 250 micron gold absorbers that have demonstrated an energy resolution of delta E_FWHM=2.3eV at an X-ray energy of 5.9keV. A similar device has shown delta E_FWHM=2.0eV at 1.5 keV. Under certain conditions and for specific device geometries, the temperature responsivity of the MPTs can vary on long timescales degrading the spectral performance. We present the characterization of different inductor geometries to optimize the design for the highest possible temperature sensitivity and compare different device designs with respect to responsivity stability.

  18. Design of High Resolution Soft X-Ray Microcalorimeters Using Magnetic Penetration Thermometers

    Science.gov (United States)

    Busch. Sarah; Balvin, Manuel; Bandler, Simon; Denis, Kevin; Finkbeiner, Fred; Porst, Jan-Patrick; Sadlier, Jack; Smith, Stephen; Stevenson, Thomas

    2012-01-01

    We have designed high-resolution soft x-ray microcalorimeters using magnetic penetration thermometers (MPTs) in an array of pixels covering a total of 2 square centimeters to have a resolving power of 300 at energies around 300 eV. This performance is desirable for studying the soft x-ray background from the warm hot intergalactic medium. MPT devices have small sensor heat capacity and high responsivities, which makes them excellent detector technology for attempting to attain sub-eV resolution. We are investigating the feasibility of pixels with absorbers that are 625 x 625 square micrometers, up to 1 x 1 square millimeters in area and 0.35 micrometer thick and thinner. Our tests have shown that suspended gold absorbers 0.35 micrometers thick (RRR = 6.7) are feasible to fabricate. We modeled the thermal diffusion from such thin gold over the size of a 625 x 625 square micrometer absorber, and conclude that the effect of the thermalization on the resolution of a 300 eV photon is an additional approximately 0.2 eV FWHM of broadening. We discuss the thermal effects of small absorber attachment sterns on solid substrate, as well as considerations for multiplexed readout. We will present the progress we have made towards building and testing this soft x-ray detector.

  19. Evidence for a resonant cyclotron line in IGR J16493-4348 from the Swift-BAT hard X-ray survey

    CERN Document Server

    D'Aì, A; La Parola, V; Segreto, A; Di Salvo, T; Iaria, R; Robba, N R; 10.1051/0004-6361/201117035

    2012-01-01

    Resonant absorption cyclotron features are a key diagnostic tool to directly measure the strength of the magnetic field of accreting neutron stars. However, typical values for cyclotron features lie in the high-energy part of the spectrum between 20 keV and 50 keV, where detection is often damped by the low statistics from single pointed observations. We show that long-term monitoring campaign performed with Swift-BAT of persistently, but faint, accreting high-mass X-ray binaries is able to reveal in their spectra the presence of cyclotron features. We extracted the average Swift-BAT 15-150 keV spectrum from the 54 months long Swift-BAT survey of the high-mass X-ray source IGR J16493-4348. To constrain the broadband spectrum we used soft X-ray spectra from Swift-XRT and Suzaku pointed observations. We model the spectra using a set of phenomenological models usually adopted to describe the energy spectrum of accreting high-mass X-ray binaries; irrespective of the models we used, we found significant improvemen...

  20. Structural and dynamical properties of chlorinated hydrocarbons studied with resonant inelastic x-ray scattering

    Science.gov (United States)

    Bohinc, R.; Žitnik, M.; Bučar, K.; Kavčič, M.; Carniato, S.; Journel, L.; Guillemin, R.; Marchenko, T.; Kawerk, E.; Simon, M.; Cao, W.

    2016-04-01

    We present a theoretical and experimental study of resonant inelastic x-ray scattering on a large group of chlorinated hydrocarbons: CH3Cl, CH2Cl2, CHCl3, CCl4, CH3CH2Cl, ClCH2CH2Cl, CH3CHCl2, CH3CCl3, C2H2Cl2-iso, C2H2Cl2-cis, C2H2Cl2-trans, and C6H5Cl. Differences in structural and dynamical properties of the molecules generated by diverse chemical environments are observed in the measured Cl(Kα) spectral maps as well as in the Cl(K) total fluorescence yield spectra. The energy position, relative intensity, and the width of the Franck-Condon distribution of low-lying σ∗ and π∗ resonances are extracted by a fitting procedure taking into account the experimental broadening. The theoretical values obtained with the transition potential and Δ Kohn-Sham methods are in good agreement with the experimental parameters indicating subtle differences due to variations in the molecular structure.

  1. Magnetic x-ray microscopy at low temperatures – Visualization of flux distributions in superconductors

    Energy Technology Data Exchange (ETDEWEB)

    Stahl, Claudia, E-mail: stahl@is.mpg.de; Ruoß, Stephen; Weigand, Markus; Bechtel, Michael; Schütz, Gisela [Max Planck Institute for Intelligent Systems, Heisenbergstraße 3, 70569 Stuttgart (Germany); Albrecht, Joachim [Research Institute for Innovative Surfaces, FINO, Aalen University, Beethovenstraße 1, 73430 Aalen (Germany)

    2016-01-28

    X-ray Magnetic Circular Dichroism (XMCD) microscopy at liquid nitrogen temperature has been performed on bilayers of high-T{sub c} superconducting YBCO (YBa{sub 2}Cu{sub 3}O{sub 7-δ}) and soft-magnetic Co{sub 40}Fe{sub 40}B{sub 20}. This should allow us to map the magnetic flux density distribution in the current-carrying state of the superconductor with high spatial resolution. For that purpose the UHV scanning X-ray microscope MAXYMUS has been upgraded by a MMR Micro Miniature Joule-Thompson cryostat capable of temperatures between 75 K and 580 K. Resulting XMCD images of the magnetic flux density in the superconductor with a field of view ranging from millimeters to micrometers are presented. The microscope’s unique combination of total electron yield (TEY) measurements together with low temperatures offers novel possibilities concerning the current transport in superconductors on small length scales.

  2. Development of low temperature and high magnetic field X-ray diffraction facility

    Energy Technology Data Exchange (ETDEWEB)

    Shahee, Aga; Sharma, Shivani; Singh, K.; Lalla, N. P., E-mail: nplallaiuc82@gmail.com; Chaddah, P. [UGC-DAE Consortium for Scientific Research, University campus, Khandwa Road, Indore-452001 (India)

    2015-06-24

    The current progress of materials science regarding multifunctional materials (MFM) has put forward the challenges to understand the microscopic origin of their properties. Most of such MFMs have magneto-elastic correlations. To investigate the underlying mechanism it is therefore essential to investigate the structural properties in the presence of magnetic field. Keeping this in view low temperature and high magnetic field (LTHM) powder x-ray diffraction (XRD), a unique state-of-art facility in the country has been developed at CSR Indore. This setup works on symmetric Bragg Brentano geometry using a parallel incident x-ray beam from a rotating anode source working at 17 kW. Using this one can do structural studies at non-ambient conditions i.e. at low- temperatures (2-300 K) and high magnetic field (+8 to −8 T). The available scattering angle ranges from 5° to 115° 2θ with a resolution better than 0.1°. The proper functioning of the setup has been checked using Si sample. The effect of magnetic field on the structural properties has been demonstrated on Pr{sub 0.5}Sr{sub 0.5}MnO{sub 3} sample. Clear effect of field induced phase transition has been observed. Moreover, the effect of zero field cooled and field cooled conditions is also observed.

  3. Effect of external resonant fields and limiter biasing on hard X-ray intensity and mirnov oscillations in IR-T1 Tokamak

    Science.gov (United States)

    Ghanbari, K.; Ghoranneviss, M.; Elahi, A. Salar

    2015-01-01

    Runaway electrons in tokamaks can cause serious damage to the first wall of the reactor and decrease its life time. Also, hard x-ray emission generated from high energy runaway electrons lead to the plasma energy loss. Therefore, suggesting methods to minimize runaway electron in tokamaks are very important. Applying external resonant field is one of the methods for controlling the Magneto Hydrodynamic (MHD) activity. Relation between the MHD activity and runaway electrons has already been studied (Jaspers et al. 1994; Ghanbari et al. 2012) Jaspers, R., et al. 1994 Phys. Rev. Lett. 72, 4093; Ghanbari, M. R., et al. 2012a Phys. Scr. 83, 055501. Present study attempts to investigate the effects of limiter biasing and Resonant Helical magnetic Field (RHF) on the generation of runaway electrons. For this purpose, plasma parameters such as plasma current, MHD oscillation, loop voltage, emitted hard x-ray intensity, Halpha impurity, safety factor in the presence and absence of external fields, were measured. Frequency activity was investigated with FFT analysis. The results show that applying resonant fields can control the MHD activity, and then hard x-ray emitted from the runaway electrons.

  4. A comparison between soft x-ray and magnetic phase data on the Madison symmetric torus

    Energy Technology Data Exchange (ETDEWEB)

    VanMeter, P. D., E-mail: pvanmeter@wisc.edu; Reusch, L. M.; Sarff, J. S.; Den Hartog, D. J. [University of Wisconsin-Madison, Madison, Wisconsin 53706 (United States); Franz, P. [Consorzio RFX, Padova (Italy)

    2016-11-15

    The Soft X-Ray (SXR) tomography system on the Madison Symmetric Torus uses four cameras to determine the emissivity structure of the plasma. This structure should directly correspond to the structure of the magnetic field; however, there is an apparent phase difference between the emissivity reconstructions and magnetic field reconstructions when using a cylindrical approximation. The difference between the phase of the dominant rotating helical mode of the magnetic field and the motion of the brightest line of sight for each SXR camera is dependent on both the camera viewing angle and the plasma conditions. Holding these parameters fixed, this phase difference is shown to be consistent over multiple measurements when only toroidal or poloidal magnetic field components are considered. These differences emerge from physical effects of the toroidal geometry which are not captured in the cylindrical approximation.

  5. Magnetic dichroism effect of binary alloys using circularly-polarized x-ray

    Energy Technology Data Exchange (ETDEWEB)

    Wu, S. Z.; Schumann, F.O.; Willis, R.F.; Goodman, K.W.; Tobin, J.G.; Carr, R.

    1997-05-01

    We have studies the magnetic propertied of CoNi binary alloy films with various atomic compositions using soft x-ray magnetic circular dichroism (XMCD) technique. The alloy films were deposited on single Cu(100) crystals in situ using our well-established epitaxial growth technique to achieve a layer-by-layer growth and a metastable fcc structure, with all films exhibiting an in-plane magnetic anistrophy. Utilizing the element-specific ability and nanostructure magnetization sensitivity of this technique, we have been able to perform the absorption measurements at L2 and L3 edge of Co and Ni atoms and observed large dichroism signals. The extraction of spin moment and orbital moment for varying elemental stoichiometry using magneto- optical sum rules is discussed.

  6. Possible detection of a cyclotron resonance scattering feature in the X-ray pulsar 4U 1909+07

    Energy Technology Data Exchange (ETDEWEB)

    Jaisawal, Gaurava K.; Naik, Sachindra [Astronomy and Astrophysics Division, Physical Research Laboratory, Ahmedabad 380009 (India); Paul, Biswajit, E-mail: gaurava@prl.res.in [Raman Research Institute, Sadashivnagar, C. V. Raman Avenue, Bangalore 560080 (India)

    2013-12-10

    We present timing and broad band spectral studies of the high-mass X-ray binary pulsar 4U 1909+07 using data from Suzaku observations during 2010 November 2-3. The pulse period of the pulsar is estimated to be 604.11 ± 0.14 s. Pulsations are seen in the X-ray light curve up to ∼70 keV. The pulse profile is found to be strongly energy-dependent: a complex, multi-peaked structure at low energy becomes a simple single peak at higher energy. We found that the 1-70 keV pulse-averaged continuum can be fit by the sum of a blackbody and a partial covering Negative and Positive power law with Exponential cutoff model. A weak iron fluorescence emission line at 6.4 keV was detected in the spectrum. An absorption-like feature at ∼44 keV was clearly seen in the residuals of the spectral fitting, independent of the continuum model adopted. To check the possible presence of a cyclotron resonance scattering feature (CRSF) in the spectrum, we normalized the pulsar spectrum with the spectrum of the Crab Nebula. The resulting Crab ratio also showed a clear dip centered at ∼44 keV. We performed statistical tests on the residuals of the spectral fitting and also on the Crab spectral ratio to determine the significance of the absorption-like feature and identified it as a CRSF of the pulsar. We estimated the corresponding surface magnetic field of the pulsar to be 3.8 × 10{sup 12} G.

  7. A setup for resonant inelastic soft x-ray scattering on liquids at free electron laser light sources

    Energy Technology Data Exchange (ETDEWEB)

    Kunnus, Kristjan; Schreck, Simon; Foehlisch, Alexander [Institute for Methods and Instrumentation for Synchrotron Radiation Research, Helmholtz-Zentrum Berlin GmbH, Albert-Einstein-Strasse 15, 12489 Berlin (Germany); Institut fuer Physik und Astronomie, Universitaet Potsdam, Karl-Liebknecht-Strasse 24/25, 14476 Potsdam (Germany); Rajkovic, Ivan; Quevedo, Wilson; Gruebel, Sebastian; Scholz, Mirko [IFG Structural Dynamics of (Bio)chemical Systems, Max Planck Institute for Biophysical Chemistry, Am Fassberg 11, 37070 Goettingen (Germany); Eckert, Sebastian; Beye, Martin; Suljoti, Edlira; Weniger, Christian; Wernet, Philippe [Institute for Methods and Instrumentation for Synchrotron Radiation Research, Helmholtz-Zentrum Berlin GmbH, Albert-Einstein-Strasse 15, 12489 Berlin (Germany); Kalus, Christian [Abteilung Betrieb Beschleuniger BESSYII, Helmholtz-Zentrum Berlin GmbH, Albert-Einstein-Strasse 15, 12489 Berlin (Germany); Nordlund, Dennis [Stanford Synchrotron Radiation Lightsource, SLAC National Accelerator Laboratory, Menlo Park, California 94025 (United States); Zhang, Wenkai; Hartsock, Robert W.; Gaffney, Kelly J. [PULSE Institute, SLAC National Accelerator Laboratory, Menlo Park, California 94025 (United States); Schlotter, William F.; Turner, Joshua J. [Linac Coherent Light Source, SLAC National Accelerator Laboratory, Menlo Park, California 94025 (United States); Kennedy, Brian [MAX-lab, PO Box 118, 221 00 Lund (Sweden); and others

    2012-12-15

    We present a flexible and compact experimental setup that combines an in vacuum liquid jet with an x-ray emission spectrometer to enable static and femtosecond time-resolved resonant inelastic soft x-ray scattering (RIXS) measurements from liquids at free electron laser (FEL) light sources. We demonstrate the feasibility of this type of experiments with the measurements performed at the Linac Coherent Light Source FEL facility. At the FEL we observed changes in the RIXS spectra at high peak fluences which currently sets a limit to maximum attainable count rate at FELs. The setup presented here opens up new possibilities to study the structure and dynamics in liquids.

  8. The space density and X-ray luminosity function of non-magnetic cataclysmic variables

    CERN Document Server

    Pretorius, Magaretha L

    2011-01-01

    We combine two complete, X-ray flux-limited surveys, the ROSAT Bright Survey (RBS) and the ROSAT North Ecliptic Pole (NEP) survey, to measure the space density (\\rho) and X-ray luminosity function (\\Phi) of non-magnetic CVs. The combined survey has a flux limit of F_X \\ga 1.1 \\times 10^{-12} erg cm^{-2}s^{-1} over most of its solid angle of just over 2\\pi, but is as deep as \\simeq 10^{-14} erg cm^{-2}s^{-1} over a small area. The CV sample that we construct from these two surveys contains 20 non-magnetic systems. We carefully include all sources of statistical error in calculating \\rho and \\Phi by using Monte Carlo simulations; the most important uncertainty proves to be the often large errors in distances estimates. If we assume that the 20 CVs in the combined RBS and NEP survey sample are representative of the intrinsic population, the space density of non-magnetic CVs is 4^{+6}_{-2} \\times 10^{-6} pc^{-3}. We discuss the difficulty in measuring \\Phi in some detail---in order to account for biases in the me...

  9. Electronic structure and characteristics of Fe 3d valence states of Fe(1.01)Se superconductors under pressure probed by x-ray absorption spectroscopy and resonant x-ray emission spectroscopy.

    Science.gov (United States)

    Chen, J M; Haw, S C; Lee, J M; Chen, S A; Lu, K T; Deng, M J; Chen, S W; Ishii, H; Hiraoka, N; Tsuei, K D

    2012-12-28

    The electronic structure and characteristics of Fe 3d valence states of iron-chalcogenide Fe(1.01)Se superconductors under pressure were probed with x-ray absorption spectroscopy and resonant x-ray emission spectroscopy (RXES). The intensity of the pre-edge peak at ~7112.7 eV of the Fe K-edge x-ray absorption spectrum of Fe(1.01)Se decreases for pressure from 0.5 GPa increased to 6.9 GPa. The satellite line Kβ' was reduced in intensity upon applying pressure and became absent for pressure 52 GPa. Fe(1.01)Se shows a small net magnetic moment of Fe(2+), likely arising from strong Fe-Fe spin fluctuations. The 1s3p-RXES spectra of Fe(1.01)Se at pressures 0.5, 6.9, and 52 GPa recorded at the Fe K-edge reveal that unoccupied Fe 3d states exhibit a delocalized character, stemming from hybridization of Fe 3d and 4p orbitals arising from a local distortion around the Fe atom in a tetrahedral site. Application of pressure causes suppression of this on-site Fe 3d-Fe 4p hybridization, and thereby decreases the intensity of the pre-edge feature in the Fe K-edge absorption spectrum of Fe(1.01)Se. Compression enhances spin fluctuations at Fe sites in Fe(1.01)Se and increases the corresponding T(c), through a competition between nearest-neighbor ferromagnetic and next-nearest-neighbor antiferromagnetic superexchange interactions. This result aids our understanding of the physics underlying iron-based superconductors.

  10. Probing single magnon excitations in Sr2IrO4 using O K-edge resonant inelastic x-ray scattering

    Science.gov (United States)

    Liu, X.; Dean, M. P. M.; Liu, J.; Chiuzbăian, S. G.; Jaouen, N.; Nicolaou, A.; Yin, W. G.; Rayan Serrao, C.; Ramesh, R.; Ding, H.; Hill, J. P.

    2015-05-01

    Resonant inelastic x-ray scattering (RIXS) at the L-edge of transition metal elements is now commonly used to probe single magnon excitations. Here we show that single magnon excitations can also be measured with RIXS at the K-edge of the surrounding ligand atoms when the center heavy metal elements have strong spin-orbit coupling. This is demonstrated with oxygen K-edge RIXS experiments on the perovskite Sr2IrO4, where low energy peaks from single magnon excitations were observed. This new application of RIXS has excellent potential to be applied to a wide range of magnetic systems based on heavy elements, for which the L-edge RIXS energy resolution in the hard x-ray region is usually poor.

  11. Combining THz laser excitation with resonant soft X-ray scattering at the Linac Coherent Light Source

    Energy Technology Data Exchange (ETDEWEB)

    Turner, Joshua J., E-mail: joshuat@slac.stanford.edu; Dakovski, Georgi L.; Hoffmann, Matthias C. [Linac Coherent Light Source, SLAC National Accelerator Laboratory, 2575 Sand Hill Road, Menlo Park, CA 94025 (United States); Hwang, Harold Y. [Department of Chemistry, Massachusetts Institute of Technology, Cambridge, MA 02139 (United States); Zarem, Alex; Schlotter, William F.; Moeller, Stefan; Minitti, Michael P. [Linac Coherent Light Source, SLAC National Accelerator Laboratory, 2575 Sand Hill Road, Menlo Park, CA 94025 (United States); Staub, Urs [Swiss Light Source, Paul Scherrer Institut, 5232 Villigen (Switzerland); Johnson, Steven [ETH Zurich, Institute for Quantum Electronics, Wolfgang-Pauli-Strasse 16, 8093 Zurich (Switzerland); Mitra, Ankush; Swiggers, Michele; Noonan, Peter; Curiel, G. Ivan; Holmes, Michael [Linac Coherent Light Source, SLAC National Accelerator Laboratory, 2575 Sand Hill Road, Menlo Park, CA 94025 (United States)

    2015-04-11

    This paper describes new instrumentation developments at the LCLS for materials studies using THz laser excitation and resonant soft X-ray scattering. This paper describes the development of new instrumentation at the Linac Coherent Light Source for conducting THz excitation experiments in an ultra high vacuum environment probed by soft X-ray diffraction. This consists of a cantilevered, fully motorized mirror system which can provide 600 kV cm{sup −1} electric field strengths across the sample and an X-ray detector that can span the full Ewald sphere with in-vacuum motion. The scientific applications motivated by this development, the details of the instrument, and spectra demonstrating the field strengths achieved using this newly developed system are discussed.

  12. A new soft X-ray magnetic circular dichroism facility at the BSRF beamline 4B7B

    CERN Document Server

    Guo, Zhi-Ying; Xing, Hai-Ying; Tang, Kun; Xui, Wei; Chen, Dong-liang; Cui, Ming-Qi; Zhao, YI-Dong

    2014-01-01

    X-ray magnetic circular dichroism (XMCD) has become an important and powerful tool because it allows the study of material properties in combination with elemental specificity, chemical state specificity, and magnetic specificity. A new soft X-ray magnetic circular dichroism apparatus has been developed at the Beijing Synchrotron Radiation Facility (BSRF). The apparatus combines three experimental conditions: ultra-high-vacuum environment, moderate magnetic fields and in-situ sample preparation to measure the absorption signal. We designed a C type dipole electromagnet that provides magnetic fields up to 0.5T in parallel (or anti-parallel) direction relative to the incoming X-ray beam. The performances of the electromagnet are measured and the results show good agreement with the simulation ones. Following film grown in situ by evaporation methods, XMCD measurements are performed. Combined polarization corrections, the magnetic moments of the Fe and Co films determined by sum rules are consistent with other t...

  13. High-resolution dichroic imaging of magnetic flux distributions in superconductors with scanning x-ray microscopy

    Energy Technology Data Exchange (ETDEWEB)

    Ruoss, Stephen; Stahl, Claudia; Weigand, Markus; Schuetz, Gisela [Max-Planck-Institut fuer Intelligente Systeme, Stuttgart (Germany); Albrecht, Joachim [Research Institute for Innovative Surfaces, FINO, Aalen University (Germany)

    2015-07-01

    The penetration of magnetic flux into the high-temperature superconductor YBCO has been observed using a new high-resolution technique based on X-ray magnetic circular dichroism (XMCD). Superconductors coated with thin soft magnetic layers of CoFeB are observed in a scanning x-ray microscope providing cooling of the sample down to 83 K under the influence of external magnetic fields. Resulting electrical currents create an inhomogeneous magnetic field distribution above the superconductor which leads to a local reorientation of the ferromagnetic layer. X-ray absorption measurements with circular polarized radiation allows the analysis of the magnetic flux distribution in the superconductor via the ferromagnetic layer. In this work we present first images taken at 83K with high spatial resolution in the nanoscale.

  14. Magnetic studies of magnetotactic bacteria by soft x-ray STXM and ptychography

    Science.gov (United States)

    Zhu, X. H.; Tyliszczak, T.; Shiu, H.-W.; Shapiro, D.; Bazylinski, D. A.; Lins, U.; Hitchcock, A. P.

    2016-01-01

    Magnetotactic bacteria (MTB) biomineralize chains of nanoscale magnetite single crystals which align the cell with the earth's magnetic field and assist the cell to migrate to, and maintain its position at, the oxic-anoxic transition zone, their preferred habitat. Here we describe use of multi-edge scanning transmission X-ray microscopy (STXM) to investigate the chemistry and magnetism of MTB on an individual cell basis. We report measurements of the orientation of the magnetic vector of magnetosome chains relative to the location of the single flagellum in marine vibrio, Magnetovibrio blakemorei strain MV-1 cells from both the southern and northern hemisphere. We also report a major improvement in both spatial resolution and spectral quality through the use of spectro-ptychography at the Fe L3 edge.

  15. High-resolution resonant inelastic soft X-ray scattering applied to liquids

    Energy Technology Data Exchange (ETDEWEB)

    Rubensson, Jan-Erik, E-mail: jan-erik.rubensson@fysik.uu.se [Department of Physics and Astronomy, Uppsala University, Box 516, S-751 20 Uppsala (Sweden); Hennies, Franz [Department of Physics and Astronomy, Uppsala University, Box 516, S-751 20 Uppsala (Sweden); MAX-lab, Lund University, Box 118, S-221 00 Lund (Sweden); Pietzsch, Annette [MAX-lab, Lund University, Box 118, S-221 00 Lund (Sweden)

    2013-06-15

    Highlights: ► Vibrational excitations in liquids resolved in RIXS are observed. ► Soft vibrational modes are quenched in the RIXS process. ► Intermolecular dipole–dipole interaction influences spectral features. ► Influence of room temperature is excitations observed. -- Abstract: The brilliance of modern synchrotron radiation sources and capabilities of new instrumentation facilitate resonant inelastic soft X-ray scattering of liquids and molecular materials with high spectral quality. Especially, when the energy resolution approaches the natural line widths a detailed analysis provides information about local potential surfaces, dynamic coupling between nuclear and electronic degrees of freedom, and intermolecular interactions. After briefly commenting on various sample handling systems we review the recent high-resolution RIXS results on liquid acetone. The experimental RIXS spectra excited at the O K edge demonstrate that the CO stretching mode dominates the vibrational progressions, and that softer modes are little affected by the nuclear dynamics in the intermediate state. It is shown that intermolecular coupling can be neglected in this specific case, and it is predicted that such interaction significantly broadens spectral features in liquids with larger dipole–dipole interaction. Analysis of the data further shows that initial state thermal excitations at room temperature have a noticeable influence on the spectral features.

  16. Quasi-particle interference of heavy fermions in resonant x-ray scattering

    Science.gov (United States)

    Gyenis, András; da Silva Neto, Eduardo H.; Sutarto, Ronny; Schierle, Enrico; He, Feizhou; Weschke, Eugen; Kavai, Mariam; Baumbach, Ryan E.; Thompson, Joe D.; Bauer, Eric D.; Fisk, Zachary; Damascelli, Andrea; Yazdani, Ali; Aynajian, Pegor

    2016-01-01

    Resonant x-ray scattering (RXS) has recently become an increasingly important tool for the study of ordering phenomena in correlated electron systems. Yet, the interpretation of RXS experiments remains theoretically challenging because of the complexity of the RXS cross section. Central to this debate is the recent proposal that impurity-induced Friedel oscillations, akin to quasi-particle interference signals observed with a scanning tunneling microscope (STM), can lead to scattering peaks in RXS experiments. The possibility that quasi-particle properties can be probed in RXS measurements opens up a new avenue to study the bulk band structure of materials with the orbital and element selectivity provided by RXS. We test these ideas by combining RXS and STM measurements of the heavy fermion compound CeMIn5 (M = Co, Rh). Temperature- and doping-dependent RXS measurements at the Ce-M4 edge show a broad scattering enhancement that correlates with the appearance of heavy f-electron bands in these compounds. The scattering enhancement is consistent with the measured quasi-particle interference signal in the STM measurements, indicating that the quasi-particle interference can be probed through the momentum distribution of RXS signals. Overall, our experiments demonstrate new opportunities for studies of correlated electronic systems using the RXS technique.

  17. d-d excitations in bilayer manganites probed by resonant inelastic x-ray scattering.

    Energy Technology Data Exchange (ETDEWEB)

    Weber, F.; Rosenkranz, S.; Castellan, J.-P.; Osborn, R.; Mitchell, J. F.; Zheng, H.; Case, D.; Kim, J. H.; Gog, T.

    2010-01-01

    We report a high-resolution resonant inelastic x-ray scattering investigation of the bilayer manganites La{sub 2-2x}Sr{sub 1+2x}Mn{sub 2}O{sub 7} with x=0.36 and 0.5. The momentum dependence along the crystallographic (110) direction for energy losses 1 eV {le} {Delta}E {le} 15 eV has been measured in detail with the data analysis focusing on the energy-loss region 1 eV {le} {Delta}E {le} 5 eV, which includes a strong peak located at {Delta}E {approx} 2 eV. We observe a clear dispersion of up to 0.5 eV in the measured q range, which is direct evidence of the nonlocal character of this excitation. Further, we found that the intensity in this low-energy region strongly depends on both the reduced wave vector q=(h,h,0), h=0.1-0.5, and temperature, i.e., different ordered phases. Results can be explained via an intersite d-d charge-transfer excitation, proposed for pseudocubic manganites, where the hopping rate is strongly increased (decreased) by ferromagnetic (antiferromagnetic) alignment of neighboring in-plane Mn ion core spins.

  18. X-ray magnetic dichroism in (Zn,Mn)O diluted magnetic semiconductors: First-principles calculations

    Science.gov (United States)

    Antonov, V. N.; Bekenov, L. V.; Mazur, D. V.; Germash, L. P.

    2012-06-01

    The electronic structure of (Zn,Mn)O diluted magnetic semiconductors was investigated theoretically from first principles by using the fully-relativistic Dirac linear muffin-tin orbital band structure method with the local spin-density approximation (LSDA) and the LSDA+ U approach. The X-ray magnetic circular dichroism (XMCD) spectra at the Mn, Zn, and O K and Mn L 2,3 edges were investigated theoretically from first principles. The origin of the XMCD spectra in these compounds was examined. The effect of oxygen vacancy atoms was found to be crucial for the X-ray magnetic dichroism at the Mn L 2,3 edges. The calculated results are compared with available experimental data.

  19. Investigations of the R5(SixGe1-x)4 Intermetallic Compounds by X-Ray Resonant Magnetic Scattering

    Energy Technology Data Exchange (ETDEWEB)

    Tan, Lizhi [Iowa State Univ., Ames, IA (United States)

    2008-08-18

    The XRMS experiment on the Gd5Ge4 system has shown that, below the Neel temperature, TN = 127 K, the magnetic unit cells is the same as the chemical unit cell. From azimuth scans and the Q dependence of the magnetic scattering, all three Gd sites in the structure were determined to be in the same magnetic space group Pnma. The magnetic moments are aligned along the c-axis and the c-components of the magnetic moments at the three different sites are equal. The ferromagnetic slabs are stacked antiferromagnetically along the b-direction. They found an unusual order parameter curve in Gd5Ge4. A spin-reorientation transition is a possibility in Gd5Ge4, which is similar to the Tb5Ge4 case. Tb5Ge4 possesses the same Sm5Ge4-type crystallographic structure and the same magnetic space group as Gd5Ge4 does. The difference in magnetic structure is that Tb5Ge4 has a canted one but Gd5Ge4 has nearly a collinear one in the low temperature antiferromagnetic phase. The competition between the magneto-crystalline anisotropy and the nearest-neighbor magnetic exchange interactions may allow a 3-dimensional canted antiferromagnetic structure in Tb5Ge4. The spin-reorientation transition in both Gd5Ge4 and Tb5Ge4 may arise from the competition between the magnetic anisotropy from the spin-orbit coupling of the conduction electrons and the dipolar interactions anisotropy.

  20. Resonant Inelastic X-ray Scattering of Rare-Earth and CopperSystems

    Energy Technology Data Exchange (ETDEWEB)

    Kvashnina, Kristina [Uppsala Univ. (Sweden)

    2007-07-11

    Rare earths and copper systems were studied using X-ray absorption spectroscopy (XAS) and resonant inelastic X-ray scattering (RIXS). The use of monochromased synchotron radiation and improved energy resolution for RIXS made possible to obtain valuable information on the electronic structure in 4f, 5f and 3d systems. Experimental results for rare-earths (Ho, Gd, Cm, U, Np, Pu) were analyzed by atomic multiplet theory based on the Hartree-Fock calculations. The inelastic scattering structures in RIXS spectra at 5d edge of actinides found to be sensitive to actinide oxidation states in different systems. Comparison of experimental and calculated Cm 5d RIXS spectra gave direct information about valency of the 248-curium isotope in oxide. Scientific understanding of processes that control chemical changes of radioactive species from spent fuel is improved by studying interactions of actinide ions (U, Np, Pu) with corroded iron surfaces. RIXS measurements at the actinide 5d edge found to be sensitive to actinide oxidation states in different systems. Comparison of experimental and calculated Cm 5d RIXS spectra gave direct information about valency of the 248 curium isotope in oxide. Scientific understanding of processes that control chemical changes of radioactive species from spent fuel is improved by studying interactions of actinide ions (U, Np, Pu) with corroded iron surfaces. RIXS measurements at the actinide 5d edge indicate the reduction of U(VI), NP(V) and Pu(VI) to U(IV), Np(IV) and Pu(IV) by presence of iron ions. This thesis is also addressed to the study of changes in the electronic structure of copper films during interaction with synthetic groundwater solutions. The surface modifications induced by chemical reactions of oxidized 100 Angstrom Cu films with CL-, SO42- and HCO3- ions in aqueous solutions with various concentrations were studied in-situ using XAS. It was shown that the pH value, the

  1. Elimination of X-Ray Diffraction through Stimulated X-Ray Transmission.

    Science.gov (United States)

    Wu, B; Wang, T; Graves, C E; Zhu, D; Schlotter, W F; Turner, J J; Hellwig, O; Chen, Z; Dürr, H A; Scherz, A; Stöhr, J

    2016-07-08

    X-ray diffractive imaging with laterally coherent x-ray free-electron laser (XFEL) pulses is increasingly utilized to obtain ultrafast snapshots of matter. Here we report the amazing disappearance of single-shot charge and magnetic diffraction patterns recorded with resonantly tuned, narrow bandwidth XFEL pulses. Our experimental results reveal the exquisite sensitivity of single-shot charge and magnetic diffraction patterns of a magnetic film to the onset of field-induced stimulated elastic x-ray forward scattering. The loss in diffraction contrast, measured over 3 orders of magnitude in intensity, is in remarkable quantitative agreement with a recent theory that is extended to include diffraction.

  2. Sum rule distortions in fluorescence-yield x-ray magnetic circular dichroism

    Science.gov (United States)

    Liu, Boyang; Piamonteze, Cinthia; Delgado-Jaime, Mario Ulises; Wang, Ru-Pan; Heidler, Jakoba; Dreiser, Jan; Chopdekar, Rajesh; Nolting, Frithjof; de Groot, Frank M. F.

    2017-08-01

    The quantitative analysis of 3 d transition metal L2 ,3 edge x-ray magnetic circular dichroism (XMCD) spectra and the related sum rules are compared for measurements with electron yield and fluorescence yield detection. Multiplet calculations on divalent ions show that fluorescence yield detected sum rule derived expectation values of Lz and Sz show noticeable deviations and detection angle dependence. We show that small deviations of the polarization dependent fluorescent decay values lead to significant deviations in the Lz and Sz sum rule values. Fe and Co experimental XMCD spectra of a supported 10 nm CoFe2O4 thin film are measured simultaneously by both electron and fluorescence yield. The deviations shown in the experimental data are well explained by the calculations and are shown to mainly depend on the polarization dependent total decay. We conclude that fluorescence yield detected x-ray magnetic circular dichroism is unsuitable for quantitative analysis of the Lz and Sz sum rule values.

  3. X-ray resonant photoexcitation: linewidths and energies of Kα transitions in highly charged Fe ions.

    Science.gov (United States)

    Rudolph, J K; Bernitt, S; Epp, S W; Steinbrügge, R; Beilmann, C; Brown, G V; Eberle, S; Graf, A; Harman, Z; Hell, N; Leutenegger, M; Müller, A; Schlage, K; Wille, H-C; Yavaş, H; Ullrich, J; Crespo López-Urrutia, J R

    2013-09-06

    Photoabsorption by and fluorescence of the Kα transitions in highly charged iron ions are essential mechanisms for x-ray radiation transfer in astrophysical environments. We study photoabsorption due to the main Kα transitions in highly charged iron ions from heliumlike to fluorinelike (Fe24+ to Fe17+) using monochromatic x rays around 6.6 keV at the PETRA III synchrotron photon source. Natural linewidths were determined with hitherto unattained accuracy. The observed transitions are of particular interest for the understanding of photoexcited plasmas found in x-ray binary stars and active galactic nuclei.

  4. Observation of Laser Induced Magnetization Dynamics in Co/Pd Multilayers with Coherent X-ray Scattering

    Energy Technology Data Exchange (ETDEWEB)

    Wu, Benny

    2012-04-05

    We report on time-resolved coherent x-ray scattering experiments of laser induced magnetization dynamics in Co/Pd multilayers with a high repetition rate optical pump x-ray probe setup. Starting from a multi-domain ground state, the magnetization is uniformly reduced after excitation by an intense 50 fs laser pulse. Using the normalized time correlation, we study the magnetization recovery on a picosecond timescale. The dynamic scattering intensity is separated into an elastic portion at length scales above 65 nm which retains memory of the initial domain magnetization, and a fluctuating portion at smaller length scales corresponding to domain boundary motion during recovery.

  5. Probing the graphite band structure with resonant soft-x-ray fluorescence

    Energy Technology Data Exchange (ETDEWEB)

    Carlisle, J.A.; Shirley, E.L.; Hudson, E.A. [Lawrence Berkeley National Lab., CA (United States)] [and others

    1997-04-01

    Soft x-ray fluorescence (SXF) spectroscopy using synchrotron radiation offers several advantages over surface sensitive spectroscopies for probing the electronic structure of complex multi-elemental materials. Due to the long mean free path of photons in solids ({approximately}1000 {angstrom}), SXF is a bulk-sensitive probe. Also, since core levels are involved in absorption and emission, SXF is both element- and angular-momentum-selective. SXF measures the local partial density of states (DOS) projected onto each constituent element of the material. The chief limitation of SXF has been the low fluorescence yield for photon emission, particularly for light elements. However, third generation light sources, such as the Advanced Light Source (ALS), offer the high brightness that makes high-resolution SXF experiments practical. In the following the authors utilize this high brightness to demonstrate the capability of SXF to probe the band structure of a polycrystalline sample. In SXF, a valence emission spectrum results from transitions from valence band states to the core hole produced by the incident photons. In the non-resonant energy regime, the excitation energy is far above the core binding energy, and the absorption and emission events are uncoupled. The fluorescence spectrum resembles emission spectra acquired using energetic electrons, and is insensitive to the incident photon`s energy. In the resonant excitation energy regime, core electrons are excited by photons to unoccupied states just above the Fermi level (EF). The absorption and emission events are coupled, and this coupling manifests itself in several ways, depending in part on the localization of the empty electronic states in the material. Here the authors report spectral measurements from highly oriented pyrolytic graphite.

  6. Chromospheric magnetic field and density structure measurements using hard X-rays in a flaring coronal loop

    CERN Document Server

    Kontar, E P; MacKinnon, A L

    2008-01-01

    A novel method of using hard X-rays as a diagnostic for chromospheric density and magnetic structures is developed to infer sub-arcsecond vertical variation of magnetic flux tube size and neutral gas density.Using Reuven Ramaty High Energy Solar Spectroscopic Imager (RHESSI) X-ray data and the newly developed X-ray visibilities forward fitting technique we find the FWHM and centroid positions of hard X-ray sources with sub-arcsecond resolution ($\\sim 0.2"$) for a solar limb flare. We show that the height variations of the chromospheric density and the magnetic flux densities can be found with unprecedented vertical resolution of $\\sim$ 150 km by mapping 18-250 keV X-ray emission of energetic electrons propagating in the loop at chromospheric heights of 400-1500 km. Our observations suggest that the density of the neutral gas is in good agreement with hydrostatic models with a scale height of around $140\\pm 30$ km. FWHM sizes of the X-ray sources decrease with energy suggesting the expansion (fanning out) of m...

  7. Theoretical analysis of the background intensity distribution in X-ray Birefringence Imaging using synchrotron bending-magnet radiation

    Energy Technology Data Exchange (ETDEWEB)

    Sutter, John P., E-mail: john.sutter@diamond.ac.uk; Dolbnya, Igor P.; Collins, Stephen P. [Diamond Light Source Ltd., Chilton, Didcot, Oxfordshire OX11 0DE (United Kingdom); Harris, Kenneth D. M.; Edwards-Gau, Gregory R. [School of Chemistry, Cardiff University, Park Place, Cardiff CF10 3AT, Wales (United Kingdom); Palmer, Benjamin A. [Department of Structural Biology, Weizmann Institute of Science, 234 Herzl St., Rehovot 7610001 (Israel)

    2015-04-28

    In the recently developed technique of X-ray Birefringence Imaging, molecular orientational order in anisotropic materials is studied by exploiting the birefringence of linearly polarized X-rays with energy close to an absorption edge of an element in the material. In the experimental setup, a vertically deflecting high-resolution double-crystal monochromator is used upstream from the sample to select the appropriate photon energy, and a horizontally deflecting X-ray polarization analyzer, consisting of a perfect single crystal with a Bragg reflection at Bragg angle of approximately 45°, is placed downstream from the sample to measure the resulting rotation of the X-ray polarization. However, if the experiment is performed on a synchrotron bending-magnet beamline, then the elliptical polarization of the X-rays out of the electron orbit plane affects the shape of the output beam. Also, because the monochromator introduces a correlation between vertical position and photon energy to the X-ray beam, the polarization analyzer does not select the entire beam, but instead selects a diagonal stripe, the slope of which depends on the Bragg angles of the monochromator and the polarization analyzer. In the present work, the final background intensity distribution is calculated analytically because the phase space sampling methods normally used in ray traces are too inefficient for this setup. X-ray Birefringence Imaging data measured at the Diamond Light Source beamline B16 agree well with the theory developed here.

  8. Theoretical analysis of the background intensity distribution in X-ray Birefringence Imaging using synchrotron bending-magnet radiation

    Science.gov (United States)

    Sutter, John P.; Dolbnya, Igor P.; Collins, Stephen P.; Harris, Kenneth D. M.; Edwards-Gau, Gregory R.; Palmer, Benjamin A.

    2015-04-01

    In the recently developed technique of X-ray Birefringence Imaging, molecular orientational order in anisotropic materials is studied by exploiting the birefringence of linearly polarized X-rays with energy close to an absorption edge of an element in the material. In the experimental setup, a vertically deflecting high-resolution double-crystal monochromator is used upstream from the sample to select the appropriate photon energy, and a horizontally deflecting X-ray polarization analyzer, consisting of a perfect single crystal with a Bragg reflection at Bragg angle of approximately 45°, is placed downstream from the sample to measure the resulting rotation of the X-ray polarization. However, if the experiment is performed on a synchrotron bending-magnet beamline, then the elliptical polarization of the X-rays out of the electron orbit plane affects the shape of the output beam. Also, because the monochromator introduces a correlation between vertical position and photon energy to the X-ray beam, the polarization analyzer does not select the entire beam, but instead selects a diagonal stripe, the slope of which depends on the Bragg angles of the monochromator and the polarization analyzer. In the present work, the final background intensity distribution is calculated analytically because the phase space sampling methods normally used in ray traces are too inefficient for this setup. X-ray Birefringence Imaging data measured at the Diamond Light Source beamline B16 agree well with the theory developed here.

  9. Modeling Flare Hard X-ray Emission from Electrons in Contracting Magnetic Islands

    Science.gov (United States)

    Guidoni, Silvina E.; Allred, Joel C.; Alaoui, Meriem; Holman, Gordon D.; DeVore, C. Richard; Karpen, Judith T.

    2016-05-01

    The mechanism that accelerates particles to the energies required to produce the observed impulsive hard X-ray emission in solar flares is not well understood. It is generally accepted that this emission is produced by a non-thermal beam of electrons that collides with the ambient ions as the beam propagates from the top of a flare loop to its footpoints. Most current models that investigate this transport assume an injected beam with an initial energy spectrum inferred from observed hard X-ray spectra, usually a power law with a low-energy cutoff. In our previous work (Guidoni et al. 2016), we proposed an analytical method to estimate particle energy gain in contracting, large-scale, 2.5-dimensional magnetic islands, based on a kinetic model by Drake et al. (2010). We applied this method to sunward-moving islands formed high in the corona during fast reconnection in a simulated eruptive flare. The overarching purpose of the present work is to test this proposed acceleration model by estimating the hard X-ray flux resulting from its predicted accelerated-particle distribution functions. To do so, we have coupled our model to a unified computational framework that simulates the propagation of an injected beam as it deposits energy and momentum along its way (Allred et al. 2015). This framework includes the effects of radiative transfer and return currents, necessary to estimate flare emission that can be compared directly to observations. We will present preliminary results of the coupling between these models.

  10. Locking of iridium magnetic moments to the correlated rotation of oxygen octahedra in Sr2IrO4 revealed by x-ray resonant scattering

    DEFF Research Database (Denmark)

    Boseggia, S.; Walker, H. C.; Vale, J.;

    2013-01-01

    Sr2IrO4 is a prototype of the class of Mott insulators in the strong spin–orbit interaction (SOI) limit described by a Jeff = 1/2 ground state. In Sr2IrO4, the strong SOI is predicted to manifest itself in the locking of the canting of the magnetic moments to the correlated rotation by 11.8(1)° o...

  11. Design and testing of planar magnetic micromotors fabricated by deep x-ray lithography and electroplating

    Energy Technology Data Exchange (ETDEWEB)

    Guckel, H.; Christenson, T.R.; Skrobis, K.J.; Klein, J. [Wisconsin Univ., Madison, WI (United States). Dept. of Electrical and Computer Engineering; Karnowsky, M. [Sandia National Labs., Albuquerque, NM (United States)

    1993-05-01

    The successful design and testing of a three-phase planar integrated magnetic micromotor is presented. Fabrication is based on a modified deep X-ray lithography and electroplating or LIGA process. Maximum rotational speeds of 33,000 rpm are obtained in air with a rotor diameter of 285 {mu}m and do not change when operated in vacuum. Real time rotor response is obtained with an integrated shaft encoder. Long lifetime is evidenced by testing to over 5(10){sup 7} ration cycles without changes in performance. Projected speeds of the present motor configuration are in the vicinity of 100 krpm and are limited by torque ripple. Higher speeds, which are attractive for sensor applications. require constant torque characteristic excitation as is evidenced by ultracentrifuge and gyroscope design. Further understanding of electroplated magnetic material properties will drive these performance improvements.

  12. Total-reflection X-ray fluorescence: An alternative tool for the analysis of magnetic ferrofluids

    Energy Technology Data Exchange (ETDEWEB)

    Fernandez-Ruiz, R. [Servicio Interdepartamental de Investigacion (SIdI), Facultad de Ciencias, Universidad Autonoma de Madrid, Cantoblanco, E-28049, Madrid (Spain)], E-mail: ramon.fernandez@uam.es; Costo, R.; Morales, M.P.; Bomati-Miguel, O.; Veintemillas-Verdaguer, S. [Instituto de Ciencia de Materiales de Madrid, CSIC, Cantoblanco, E-28049, Madrid (Spain)

    2008-12-15

    This work presents the first application of the total-reflection X-ray fluorescence (TXRF) to the compositional study of magnetic ferrofluids. With the aims of validating the best analytical conditions and also, limitations of the TXRF in the compositional study of these materials, an alternative empirical method, based in the use of angle-dependence TXRF (AD-TXRF) measurements, is proposed. Three kinds of ferromagnetic nanoparticles, with different morphologies, have been studied. The techniques of inductively coupled plasma mass spectrometry (ICP-MS) and inductively coupled plasma optical emission spectroscopy (ICP-OES) have been used to validate the TXRF results. In contrast with the plasma techniques, the developed TXRF procedure need not of previous chemical acid digestion. Additionally, two procedures of magnetic nanoparticles synthesis, co-precipitation and laser-pyrolysis, have been checked for the contaminants trace metals Zn, Mn and Cr. It has been found that the method of laser-pyrolysis produces nanoparticles of higher purity.

  13. Modelling X-ray emitting stationary shocks in magnetized protostellar jets

    Science.gov (United States)

    Ustamujic, S.; Orlando, S.; Bonito, R.; Miceli, M.; Gómez de Castro, A. I.; López-Santiago, J.

    2017-03-01

    The early stages of a star birth are characterized by a variety of mass ejection phenomena, including outflows and collimated jets that are strongly related to the accretion process developed in the context of the star-disc interaction. Jets move through the ambient medium producing complex structures observed at different wavelengths. In particular, X-ray observations show evidence of strong shocks heating the plasma up to a few million degrees. In some cases, the shocked features appear to be stationary. They are interpreted as shock diamonds. We aim at investigating the physical properties of the shocked plasma and the role of magnetic fields on the collimation of the jet and the formation of a stationary shock. We performed 2.5D MHD simulations modelling the propagation of a jet ramming with a supersonic speed into an initially isothermal and homogeneous magnetized medium and compared the results with observations.

  14. Lateral spin transfer torque induced magnetic switching at room temperature demonstrated by x-ray microscopy.

    Science.gov (United States)

    Buhl, M; Erbe, A; Grebing, J; Wintz, S; Raabe, J; Fassbender, J

    2013-01-01

    Changing and detecting the orientation of nanomagnetic structures, which can be used for durable information storage, needs to be developed towards true nanoscale dimensions for keeping up the miniaturization speed of modern nanoelectronic components. Therefore, new concepts for controlling the state of nanomagnets are currently in the focus of research in the field of nanoelectronics. Here, we demonstrate reproducible switching of a purely metallic nanopillar placed on a lead that conducts a spin-polarized current at room temperature. Spin diffusion across the metal-metal (Cu to CoFe) interface between the pillar and the lead causes spin accumulation in the pillar, which may then be used to set the magnetic orientation of the pillar. In our experiments, the detection of the magnetic state of the nanopillar is performed by direct imaging via scanning transmission x-ray microscopy (STXM).

  15. Lateral spin transfer torque induced magnetic switching at room temperature demonstrated by x-ray microscopy

    Science.gov (United States)

    Buhl, M.; Erbe, A.; Grebing, J.; Wintz, S.; Raabe, J.; Fassbender, J.

    2013-01-01

    Changing and detecting the orientation of nanomagnetic structures, which can be used for durable information storage, needs to be developed towards true nanoscale dimensions for keeping up the miniaturization speed of modern nanoelectronic components. Therefore, new concepts for controlling the state of nanomagnets are currently in the focus of research in the field of nanoelectronics. Here, we demonstrate reproducible switching of a purely metallic nanopillar placed on a lead that conducts a spin-polarized current at room temperature. Spin diffusion across the metal-metal (Cu to CoFe) interface between the pillar and the lead causes spin accumulation in the pillar, which may then be used to set the magnetic orientation of the pillar. In our experiments, the detection of the magnetic state of the nanopillar is performed by direct imaging via scanning transmission x-ray microscopy (STXM). PMID:24126435

  16. Soft gamma-ray repeaters and anomalous X-ray pulsars as highly magnetized white dwarfs

    CERN Document Server

    Mukhopadhyay, Banibrata

    2016-01-01

    We explore the possibility that soft gamma-ray repeaters (SGRs) and anomalous X-ray pulsars (AXPs) are powered by highly magnetized white dwarfs (B-WDs). We take a sample of SGRs and AXPs and provide the possible parameter space in mass, radius, and surface magnetic field based on their observed properties (period and its derivative) and the assumption that these sources obey the mass-radius relation derived for the B-WDs. The radius and magnetic field of B-WDs are adequate to explain energies in SGRs/AXPs as the rotationally powered energy. In addition, B-WDs also adequately explain the perplexing radio transient GCRT J1745-3009 as a white dwarf pulsar. Note that the radius and magnetic fields of B-WDs are neither extreme (unlike of highly magnetized neutron stars) nor ordinary (unlike of magnetized white dwarfs, yet following the Chandrasekhar's mass-radius relation (C-WDs)). In order to explain SGRs/AXPs, while the highly magnetized neutron stars require an extra, observationally not well established yet, ...

  17. Studying nanomagnets and magnetic heterostructures with X-ray PEEM at the Swiss Light Source

    Energy Technology Data Exchange (ETDEWEB)

    Le Guyader, Loiec; Kleibert, Armin [Swiss Light Source, Paul Scherrer Institut, 5232 Villigen PSI (Switzerland); Fraile Rodriguez, Arantxa [Departament de Fisica Fonamental and Institut de Nanociencia i Nanotecnologia (IN2UB), Universitat de Barcelona, 08028 Barcelona (Spain); El Moussaoui, Souliman; Balan, Ana; Buzzi, Michele; Raabe, Joerg [Swiss Light Source, Paul Scherrer Institut, 5232 Villigen PSI (Switzerland); Nolting, Frithjof, E-mail: frithjof.nolting@psi.ch [Swiss Light Source, Paul Scherrer Institut, 5232 Villigen PSI (Switzerland)

    2012-10-15

    Highlights: Black-Right-Pointing-Pointer Time resolved PEEM set up using a femtosecond laser as the pump pulse. Black-Right-Pointing-Pointer Magnetization vectometry based on advanced computer algorithms enables the determination of the in-plane and out-of-plane magnetization directions in micro and nanostructures. Black-Right-Pointing-Pointer Special sample holders allow measurements in applied magnetic fields to study the hysteresis loop of nanoparticles and to image in up to 40 mT out-of-plane magnetic fields. -- Abstract: Polarization dependent X-ray absorption spectroscopy and microscopy enables the element selective investigation of magnetic systems at the nanoscale. At the Swiss Light Source a photoemission electron microscope is used for the study of a broad variety of systems. Here, a review of recent activities is presented with a focus on instrumental and analytical developments. A new procedure for the 3 dimensional determination of the magnetization vector has been developed, and is demonstrated for GdFeCo microstructures displaying in-plane and out-of-plane domains, and sub-20 nm Fe nanoparticles. The recent progress for measurements in applied magnetic fields is presented and a new set-up for time-resolved measurements employing femtosecond laser pulses is described.

  18. Soft gamma-ray repeaters and anomalous X-ray pulsars as highly magnetized white dwarfs

    Science.gov (United States)

    Mukhopadhyay, Banibrata; Rao, A. R.

    2016-05-01

    We explore the possibility that soft gamma-ray repeaters (SGRs) and anomalous X-ray pulsars (AXPs) are powered by highly magnetized white dwarfs (B-WDs). We take a sample of SGRs and AXPs and provide the possible parameter space in mass, radius, and surface magnetic field based on their observed properties (period and its derivative) and the assumption that these sources obey the mass-radius relation derived for the B-WDs. The radius and magnetic field of B-WDs are adequate to explain energies in SGRs/AXPs as the rotationally powered energy. In addition, B-WDs also adequately explain the perplexing radio transient GCRT J1745-3009 as a white dwarf pulsar. Note that the radius and magnetic fields of B-WDs are neither extreme (unlike of highly magnetized neutron stars) nor ordinary (unlike of magnetized white dwarfs, yet following the Chandrasekhar's mass-radius relation (C-WDs)). In order to explain SGRs/AXPs, while the highly magnetized neutron stars require an extra, observationally not well established yet, source of energy, the C-WDs predict large ultra-violet luminosity which is observationally constrained from a strict upper limit. Finally, we provide a set of basic differences between the magnetar and B-WD hypotheses for SGRs/AXPs.

  19. Nanoscale thermal, acoustic, and magnetic dynamics probed with soft x-ray light

    Science.gov (United States)

    Siemens, Mark E.

    This thesis discusses the application of coherent, ultrafast beams of soft x-ray light from high-order harmonic generation (HHG) to study thermal, acoustic, and magnetic processes in nanostructures. This short-wavelength light is a uniquely powerful probe of surface dynamics since it has both a very short wavelength and duration. First, this thesis reports the first observation and quantitative measurements of the transition from diffusive to ballistic thermal transport for the case of heat flow away from a heated nanostructure into a bulk substrate. This measurement provides insight into the fundamentals of thermal energy transport away from nanoscale hot spots, and demonstrates a fundamental limit to the energy dissipation capability of nanostructures. Further, we propose a straightforward correction to the Fourier law for heat diffusion, necessary for thermal management in nanoelectronics, nano-enabled energy systems, nanomanufacturing, and nanomedicine. Second, this work discusses dynamic measurements of ultra-high frequency surface acoustic waves (SAW) and the first SAW dispersion measurement in a nanostructured system. These results are directly applicable to adhesion and thickness diagnostics of very thin films. Finally, this thesis reports the first use of light from HHG to study magnetic orientation. Using the transverse magneto-optic Kerr effect and soft x-ray light near the M-absorption edges of Fe, Co, and Ni, magnetic asymmetries up to 8% are observed from thin Permalloy (Ni80Fe20) films. This signal is 1-2 orders of magnitude higher than that observed using optical methods, showing great promise for dynamic imaging of domain flipping at the 100 nm level.

  20. Data Mining Solar X-Ray Flares Triggered by Emerging Magnetic Flux

    Science.gov (United States)

    Loftus, Kaitlyn; Saar, Steven H.; Schanche, Nicole

    2017-01-01

    We investigate the association between emerging magnetic flux and solar X-ray flares to identify, and if possible quantify, distinguishing physical properties of flares triggered by flux emergence versus those triggered by other sources. Our study uses as its basis GOES-classified solar flares from March 2011 through June 2016 that have been identified by the Space Weather Prediction Center’s flare detection algorithm. The basic X-ray flare data is then enriched with data about related EUV-spectrum flares, emerging fluxes, active regions, eruptions, and sigmoids, which are all characterized by event-specific keywords, identified via SDO feature finding tools, and archived in the Heliophysics Events Knowledgebase (HEK). Using appropriate spatial and temporal parameters for each event type to determine association, we create a catalogue of solar events associated with each GOES-classified flare. After accounting for the primitive state of many of these event detection algorithms, we statistically analyze the compiled dataset to determine the effects of an emerging flux trigger on flare properties. A two-sample Kolmogorov-Smirnov test confirms with 99.9% confidence that flares triggered by emerging flux have a different peak flux distribution than non-emerging-flux-associated flares. We observe no linear or logarithmic correlations between flares’ and their associated emerging fluxes’ individual properties and find flares triggered by emerging flux are ~ 10% more likely to cause an eruption inside an active region while outside of an active region, the flare’s association with emerging flux has no effect on its likeliness to cause an eruption. We also compare the morphologies of the flares triggered by emerging flux and flares not via a superposed epoch analysis of lightcurves. Our results will be of interest for predicting flare behavior as a function of magnetic activity (where we can use enhanced rates of emerging flux as a proxy for heightened stellar

  1. Renormalization Group Approach to the X-Ray Absorption Problem and Application to the Vigman-Finkelshtein Model for Magnetic Impurities in Metals.

    Science.gov (United States)

    Nunes de Oliveira, Luiz

    The renormalization group techniques developed by Wilson for the Kondo problem are applied to three related problems: the absorption of x-rays by metals, the absorption of x-rays by impurities in metals, and the specific heat of dilute magnetic alloys. In the first problem considered, the x-ray absorption problem, the metal is represented by a half-filled conduction band and a deep level representing a core state. The absorption of an x-ray photon excites an electron from this core level to the conduction band creating a core hole whose positive charge interacts with the conduction electrons. The absorption spectrum is, for the first time, calculated in the energy range 10('-10)D ) (omega)(,T)) expression to seven decimal places; the prefactor (mu)(,o) is calculated for the first time. For (omega)-(omega)(,T) (TURNEQ) D, remarkably small deviations (e.g., deviations of 15% for (omega)-(omega)(,T) = .3D) from the Nozieres-De Dominicis power law are found. As a second application of the renormalization group techniques, the x-ray absorption spectrum for the resonant level model for impurities in metals is calculated. In this model, the metal is represented by a half-filled conduction band and the impurity by two levels: a core level from which an electron is excited to the conduction band by the absorption of an x-ray photon, and a resonant level, coupled to the conduction electrons, whose energy is lowered by the interaction with the core hole created by the absorption of the x-ray. In the x-ray absorption process, the resonant level is thus shifted to lower energy. The absorption spectrum approaches a power law in the energy range (omega)-(omega)(,T) >> (GAMMA), where (GAMMA) is the width of the resonant level, and a different power law in the range (omega)-(omega)(,T) body effect found in the spectrum of certain systems having a discrete level coupled to a continuum of energies) is elaborated. The problem of the specific heat of dilute magnetic alloys is attacked

  2. Closed bore XMR (CBXMR) systems for aortic valve replacement: Active magnetic shielding of x-ray tubes

    Energy Technology Data Exchange (ETDEWEB)

    Bracken, John A.; DeCrescenzo, Giovanni; Komljenovic, Philip; Lillaney, Prasheel V.; Fahrig, Rebecca; Rowlands, J. A. [Department of Medical Biophysics and Sunnybrook Health Sciences Center, University of Toronto, 2075 Bayview Avenue, Toronto, Ontario M4N 3M5 (Canada); Department of Radiology, Stanford University, Stanford, California 94305 (United States); Department of Medical Biophysics and Sunnybrook Health Sciences Center, University of Toronto, 2075 Bayview Avenue, Toronto, Ontario M4N 3M5 (Canada)

    2009-05-15

    Hybrid closed bore x-ray/MRI systems are being developed to improve the safety and efficacy of percutaneous aortic valve replacement procedures by harnessing the complementary strengths of the x-ray and MRI modalities in a single interventional suite without requiring patient transfer between two rooms. These systems are composed of an x-ray C-arm in close proximity ({approx_equal}1 m) to an MRI scanner. The MRI magnetic fringe field can cause the electron beam in the x-ray tube to deflect. The deflection causes the x-ray field of view to shift position on the detector receptacle. This could result in unnecessary radiation exposure to the patient and the staff in the cardiac catheterization laboratory. Therefore, the electron beam deflection must be corrected. The authors developed an active magnetic shielding system that can correct for electron beam deflection to within an accuracy of 5% without truncating the field of view or increasing exposure to the patient. This system was able to automatically adjust to different field strengths as the external magnetic field acting on the x-ray tube was changed. Although a small torque was observed on the shielding coils of the active shielding system when they were placed in a magnetic field, this torque will not impact their performance if they are securely mounted on the x-ray tube and the C-arm. The heating of the coils of the shielding system for use in the clinic caused by electric current was found to be slow enough not to require a dedicated cooling system for one percutaneous aortic valve replacement procedure. However, a cooling system will be required if multiple procedures are performed in one session.

  3. CALCULATION OF MAGNETIC-X-RAY DICHROISM IN 4D AND 5D ABSORPTION-SPECTRA OF ACTINIDES

    NARCIS (Netherlands)

    OGASAWARA, H; KOTANI, A; THOLE, BT

    1991-01-01

    We present atomic calculations of the magnetic dichroism in 4d and 5d x-ray-absorption (XAS) spectra of trivalent actinide ions. The calculations are carried out for both linearly and circularly polarized light at zero temperature. Large magnetic dichroism is predicted for 5d XAS with

  4. X-ray and magnetic studies of Zn2+ substituted Ni–Pb ferrites

    Indian Academy of Sciences (India)

    M C Sable; B K Labde; N R Shamkuwar

    2005-02-01

    Seven samples of the polycrystalline, Ni1.25–ZnPb0.25Fe1.5O4 ( = 0.0, 0.1, 0.2, 0.3, 0.4, 0.5 and 0.6) ferrites, were prepared by usual double sintering ceramic method. X-ray diffraction patterns of the samples revealed single-phase cubic spinel structure. The magnetic properties were investigated by means of magnetization and a.c. susceptibility () measurements. A.C. susceptibility was measured from room temperature to the Curie temperature (C) of the samples. Variation of a.c. susceptibility () with temperature showed that the samples with = 0.3 and 0.5 contain single-domain (SD) particles whereas the samples with = 0.4 and 0.6 showed multi-domain (MD) nature. Values of Curie temperature (C) as obtained from the study of variation of a.c. susceptibility with temperature were found to decrease with increase in the Zn2+ concentration (). Magnetic measurements showed increase in magnetization as Zn2+ content was increased from 0.0 to 0.5. Further increase in Zn2+ content () reduces the magnetization.

  5. Collimating Montel mirror as part of a multi-crystal analyzer system for resonant inelastic x-ray scattering

    Energy Technology Data Exchange (ETDEWEB)

    Kim, Jungho; Shi, Xianbo; Casa, Diego; Qian, Jun; Huang, XianRong; Gog, Thomas

    2016-07-01

    Advances in resonant inelastic x-ray scattering (RIXS) have come in lockstep with improvements in energy resolution. Currently, the best energy resolution at the Ir-L3 edge stands at ~25 meV, which is achieved using a diced Si spherical analyzer. An angular dispersion analyzer system using multiple flat crystals provides a promising way to achieve higher energy resolution, namely 10 meV or better, thereby overcoming the intrinsic energy resolution limit of diced spherical crystal analyzers. One essential component for a practical use of such multi-crystal systems is the xray collimation optics. In this work, a laterally graded, parabolic collimation Montel mirror was designed with larger than 10 mrad acceptance, collimating the x-ray beam to smaller than 100 μrad divergence at the Ir-L3 absorption energy. The x-ray collimation performance was investigated at beamline 27-ID of the Advanced Photon Source, using incident photons from a Diamond (111) monochromator illuminating a controlled 40 mrad divergence scattering source of 5 μm diameter. A flat Si (111) crystal served as the analyzer. It is found from experimental data and ray-tracing simulations, combined with metrology results, that the manufactured Montel mirror satisfies the required specifications of angular acceptance and collimated x-ray divergence for a high resolution RIXS spectrometer at the Ir-L3 edge.

  6. Arsenic speciation by X-ray spectroscopy using resonant Raman Scattering

    Energy Technology Data Exchange (ETDEWEB)

    Sanchez, H.J.; Leani, J.J. [Universidad Nacional de Cordoba, Cba (Argentina); Perez, C.A. [Laboratorio Nacional de Luz Sincrotron (LNLS), Campinas, SP (Brazil)

    2012-07-01

    Full text: The toxicity of arsenic species is widely known. A realistic evaluation of the risk posed by As depends on accurate determination of As speciation, because its toxicity and mobility varies with oxidation state and chemical environment. The most toxic species are inorganic As (III) and As (V) called respectively arsenite or trivalent arsenic, and arsenate or pentavalent arsenic. Recently, x-ray Resonant Raman Scattering spectroscopy has been successfully employed to determine the oxidation state of metals. In this work we use RRS spectroscopy to perform arsenic speciation. The measurements were carried out in XRF station of the D09B-XRF beamline at the Brazilian synchrotron facility (LNLS, Campinas). Mineral samples of As in different oxidation states (As(III) and AS(V)), and two biological forms of arsenic (monomethylarsonic acid (MMA(V) and dimethylarsinic acid DMA(V)) were analysed. The samples were diluted, deposited on silicon wafers and allowed to dry. The amount of liquid deposited on the reflector before evaporation was 20 microliters for all the specimens. These samples were irradiated with monochromatic photons of 11816 eV, i.e., below the K-edge of arsenic in order to inspect the Raman emissions. The measuring lifetime was 3600 sec for each sample. Spectra were analysed with specific programs for spectrum analysis using non-conventional functions for data fitting, i.e., modified Voight functions (for Compton peaks), Gaussian functions for fluorescent and for low intensity peaks (such as escape peaks and other contributions), and polynomial functions for the background. Raman peaks were fitted using specific functions. In this work we have shown that resonant Raman scattering spectroscopy can be used to analyse arsenic species. The method is very simple and reliable. The most important feature of this method relies in the possibility of using the same spectrometer of XRF analysis or TXRF analysis. In this way, practically in the same experiment

  7. A gamma- and X-ray detector for cryogenic, high magnetic field applications

    CERN Document Server

    Cooper, R L; Bales, M J; Bass, C D; Beise, E J; Breuer, H; Byrne, J; Chupp, T E; Coakley, K J; Dewey, M S; Fu, C; Gentile, T R; Mumm, H P; Nico, J S; O'Neill, B; Pulliam, K; Thompson, A K; Wietfeldt, F E

    2012-01-01

    As part of an experiment to measure the spectrum of photons emitted in beta-decay of the free neutron, we developed and operated a detector consisting of 12 bismuth germanate (BGO) crystals coupled to avalanche photodiodes (APDs). The detector was operated near liquid nitrogen temperature in the bore of a superconducting magnet and registered photons with energies from 5 keV to 1000 keV. To enlarge the detection range, we also directly detected soft X-rays with energies between 0.2 keV and 20 keV with three large area APDs. The construction and operation of the detector is presented, as well as information on operation of APDs at cryogenic temperatures.

  8. Analytical modelling and x-ray imaging of oscillations of a single magnetic domain wall

    Energy Technology Data Exchange (ETDEWEB)

    Bocklage, Lars; Kruger, Benjamin; Fischer, Peter; Meier, Guido

    2009-07-10

    Domain-wall oscillation in a pinnig potential is described analytically in a one dimensional model for the feld-driven case. For a proper description the pinning potential has to be extended by nonharmonic contributions. Oscillations of a domain wall are observed on its genuine time scale by magnetic X-ray microscopy. It is shown that the nonharmonic terms are present in real samples with a strong restoring potential. In the framework of our model we gain deep insight into the domain-wall motion by looking at different phase spaces. The corrections of the harmonic potential can change the motion of the domain wall significantly. The damping parameter of permalloy is determined via the direct imaging technique.

  9. An ultrahigh-vacuum apparatus for resonant diffraction experiments using soft x rays (hnu=300-2000 eV).

    Science.gov (United States)

    Takeuchi, T; Chainani, A; Takata, Y; Tanaka, Y; Oura, M; Tsubota, M; Senba, Y; Ohashi, H; Mochiku, T; Hirata, K; Shin, S

    2009-02-01

    We have developed an ultrahigh-vacuum instrument for resonant diffraction experiments using polarized soft x rays in the energy range of hnu=300-2000 eV at beamline BL17SU of SPring-8. The diffractometer consists of modified differentially pumped rotary feedthroughs for theta-2theta stages, a sample manipulator with motor-controlled x-y-z-, tilt (chi)-, and azimuth (phi)-axes, and a liquid helium flow-type cryostat for temperature dependent measurements between 30 and 300 K. Test results indicate that the diffractometer exhibits high reproducibility (better than 0.001 degrees ) for a Bragg reflection of alpha-quartz 100 at a photon energy of hnu=1950 eV. Typical off- and on-resonance Bragg reflections in the energy range of 530-1950 eV could be measured using the apparatus. The results show that x-ray diffraction experiments with energy-, azimuth-, and incident photon polarization-dependence can be reliably measured using soft x rays in the energy range of approximately 300-2000 eV. The facility can be used for resonant diffraction experiments across the L-edge of transition metals, M-edge of lanthanides, and up to the Si K-edge of materials.

  10. The role of the disk magnetization on the hysteresis behavior of X-ray binaries

    CERN Document Server

    Petrucci, P O; Henri, G; Pelletier, G

    2007-01-01

    We present a framework for understanding the dynamical and spectral properties of X-ray Binaries, where the presence of an organized large scale magnetic field plays a major role. Such a field is threading the whole accretion disk with an amplitude measured by the disk magnetization $\\mu(r,t) =B_z^2/(\\mu_o P_{tot})$, where $P_{tot}$ is the total, gas and radiation, pressure. Below a transition radius $r_J$, a jet emitting disk (the JED) is settled and drives self-collimated non relativistic jets. Beyond $r_J$, no jet is produced despite the presence of the magnetic field and a standard accretion disc (the SAD) is established. The radial distribution of the disk magnetization $\\mu$ adjusts itself to any change of the disk accretion rate $\\dot m$, thereby modifying the transition radius $r_J$. We propose that a SAD-to-JED transition occurs locally, at a given radius, in a SAD when $\\mu=\\mu_{max} \\simeq 1$ while the reverse transition occurs in a JED only when $\\mu=\\mu_{min}\\simeq 0.1$. This bimodal behavior of ...

  11. Fast and slow magnetic deflagration fronts in Type I X-ray bursts

    CERN Document Server

    Cavecchi, Yuri; Watts, Anna L; Braithwaite, Jonathan

    2015-01-01

    Type I X-ray bursts are produced by thermonuclear runaways that develop on accreting neutron stars. Once one location ignites, the flame propagates across the surface of the star. Flame propagation is fundamental in order to understand burst properties like rise time and burst oscillations. Previous work quantified the effects of rotation on the front, showing that the flame propagates as a deflagration and that the front strongly resembles a hurricane. However the effect of magnetic fields was not investigated, despite the fact that magnetic fields strong enough to have an effect on the propagating flame are expected to be present on many bursters. In this paper we show how the coupling between fluid layers introduced by an initially vertical magnetic field plays a decisive role in determining the character of the fronts that are responsible for the Type I bursts. In particular, on a star spinning at 450 Hz (typical among the bursters) we test seed magnetic fields of $10^{7} - 10^{10}$ G and find that for th...

  12. Development of Position-Sensitive Magnetic Calorimeters for X-Ray Astronomy

    Science.gov (United States)

    Bandler, SImon; Stevenson, Thomas; Hsieh, Wen-Ting

    2011-01-01

    Metallic magnetic calorimeters (MMC) are one of the most promising devices to provide very high energy resolution needed for future astronomical x-ray spectroscopy. MMC detectors can be built to large detector arrays having thousands of pixels. Position-sensitive magnetic (PoSM) microcalorimeters consist of multiple absorbers thermally coupled to one magnetic micro calorimeter. Each absorber element has a different thermal coupling to the MMC, resulting in a distribution of different pulse shapes and enabling position discrimination between the absorber elements. PoSMs therefore achieve the large focal plane area with fewer number of readout channels without compromising spatial sampling. Excellent performance of PoSMs was achieved by optimizing the designs of key parameters such as the thermal conductance among the absorbers, magnetic sensor, and heat sink, as well as the absorber heat capacities. Micro fab ri - cation techniques were developed to construct four-absorber PoSMs, in which each absorber consists of a two-layer composite of bismuth and gold. The energy resolution (FWHM full width at half maximum) was measured to be better than 5 eV at 6 keV x-rays for all four absorbers. Position determination was demonstrated with pulse-shape discrimination, as well as with pulse rise time. X-ray microcalorimeters are usually designed to thermalize as quickly as possible to avoid degradation in energy resolution from position dependence to the pulse shapes. Each pixel consists of an absorber and a temperature sensor, both decoupled from the cold bath through a weak thermal link. Each pixel requires a separate readout channel; for instance, with a SQUID (superconducting quantum interference device). For future astronomy missions where thousands to millions of resolution elements are required, having an individual SQUID readout channel for each pixel becomes difficult. One route to attaining these goals is a position-sensitive detector in which a large continuous or

  13. Burn out or fade away? On the X-ray and magnetic death of intermediate mass stars

    Energy Technology Data Exchange (ETDEWEB)

    Drake, Jeremy J.; Kashyap, Vinay; Günther, H. Moritz; Wright, Nicholas J. [Smithsonian Astrophysical Observatory, MS-3, 60 Garden Street, Cambridge, MA 02138 (United States); Braithwaite, Jonathan, E-mail: jdrake@cfa.harvard.edu [Argelander Institut für Astronomie, Auf dem Hügel 71, D-53121 Bonn (Germany)

    2014-05-10

    The nature of the mechanisms apparently driving X-rays from intermediate mass stars lacking strong convection zones or massive winds remains poorly understood, and the possible role of hidden, lower mass close companions is still unclear. A 20 ks Chandra HRC-I observation of HR 4796A, an 8 Myr old main sequence A0 star devoid of close stellar companions, has been used to search for a signature or remnant of magnetic activity from the Herbig Ae phase. X-rays were not detected and the X-ray luminosity upper limit was L{sub X} ≤ 1.3 × 10{sup 27} erg s{sup –1}. The result is discussed in the context of various scenarios for generating magnetic activity, including rotational shear and subsurface convection. A dynamo driven by natal differential rotation is unlikely to produce observable X rays, chiefly because of the difficulty in getting the dissipated energy up to the surface of the star. A subsurface convection layer produced by the ionization of helium could host a dynamo that should be effective throughout the main sequence but can only produce X-ray luminosities of the order 10{sup 25} erg s{sup –1}. This luminosity lies only moderately below the current detection limit for Vega. Our study supports the idea that X-ray production in Herbig Ae/Be stars is linked largely to the accretion process rather than the properties of the underlying star, and that early A stars generally decline in X-ray luminosity at least 100,000 fold in only a few million years.

  14. Resonant X-ray scattering study on the filled skutterudite PrFe{sub 4}P{sub 12}

    Energy Technology Data Exchange (ETDEWEB)

    Ishii, K.; Inami, T.; Murakami, Y.; Hao, L.; Iwasa, K.; Kohgi, M.; Aoki, Y.; Sugawara, H.; Sato, H.; Imada, S.; Nakao, H.; Sawa, H.; Wakabayashi, Y

    2003-05-01

    Resonant X-ray scattering study was carried out to investigate an anomalous ordered state (T{sub A}=6.5 K) in the filled skutterudite PrFe{sub 4}P{sub 12}. At the Pr-L{sub III} absorption edge, we observed resonant features in h+k+l=odd reflections, which are forbidden in the BCC structure above T{sub A}. Because these reflections contain the difference of anomalous scattering factor between two Pr atoms in the BCC unit cell, and the ordered state is attributed to the ordering of two different electronic states of Pr.

  15. A study of magnetic moments of CeRh3B2 by X-ray magnetic diffraction experiments

    Science.gov (United States)

    Ito, M.; Suzuki, K.; Tadenuma, T.; Nagayasu, R.; Sakurai, Y.; Onuki, Y.; Nishibori, E.; Sakata, M.

    2014-04-01

    X-ray magnetic diffraction experiments of a ferromagnetic rare-earth compound CeRh3B2 have been performed, and the spin and orbital magnetic form factors have been measured. Density distributions of the spin and orbital magnetic moments in real space have been obtained by using Maximum Entropy Method. Low peaks at Rh sites as well as high peaks at Ce sites are observed in these distribution maps. We have estimated the spin and orbital magnetic moments at the Ce and Rh sites in the distribution maps, and have obtained small but nonnegligible spin and orbital magnetic moments of Rh. This is probably the first experimental evidence showing existence of the spin and orbital moments of Rh in this compound.

  16. Resonant x-ray emission spectroscopy of liquid water: novel instrumentation, high resolution, and the"map" approach

    Energy Technology Data Exchange (ETDEWEB)

    Weinhardt, L.; Fuchs, O.; Blum, M.; B& #228; r, M.; Weigand, M.; Denlinger, J.D.; Zubavichus, Y.; Zharnikov, M.; Grunze, M.; Heske, C.; Umbach, E.

    2008-06-17

    Techniques to study the electronic structure of liquids are rare. Most recently, resonant x-ray emission spectroscopy (XES) has been shown to be an extremely versatile spectroscopy to study both occupied and unoccupied electronic states for liquids in thermodynamic equilibrium. However, XES requires high-brilliance soft x-ray synchrotron radiation and poses significant technical challenges to maintain a liquid sample in an ultra-high vacuum environment. Our group has therefore developed and constructed a novel experimental setup for the study of liquids, with the long-term goal of investigating the electronic structure of biological systems in aqueous environments. We have developed a flow-through liquid cell in which the liquid is separated from vacuum by a thin Si3N4 or SiC window and which allows a precise control of temperature. This approach has significant advantages compared to static liquids cells used in the past. Furthermore, we have designed a dedicated high-transmission, high-resolution soft x-ray spectrometer. The high transmission makes it possible to measure complete resonant XES"maps" in less than an hour, giving unprecedented detailed insight into the electronic structure of the investigated sample. Using this new equipment we have investigated the electronic structure of liquid water. Furthermore, our XES spectra and maps give information about ultra-fast dissociation on the timescale of the O 1s core hole lifetime, which is strongly affected by the initial state hydrogen bonding configuration.

  17. Magnetism at spinel thin film interfaces probed through soft x-ray spectroscopy techniques

    Energy Technology Data Exchange (ETDEWEB)

    Chopdekar, R.V.; Liberati, M.; Takamura, Y.; Kourkoutis, L. Fitting; Bettinger, J. S.; Nelson-Cheeseman, B. B.; Arenholz, E.; Doran, A.; Scholl, A.; Muller, D. A.; Suzuki, Y.

    2009-12-16

    Magnetic order and coupling at the interfaces of highly spin polarized Fe{sub 3}O{sub 4} heterostructures have been determined by surface sensitive and element specific soft x-ray spectroscopy and spectromicroscopy techniques. At ambient temperature, the interface between paramagnetic CoCr{sub 2}O{sub 4} or MnCr{sub 2}O{sub 4} and ferrimagnetic Fe{sub 3}O{sub 4} isostructural bilayers exhibits long range magnetic order of Co, Mn and Cr cations which cannot be explained in terms of the formation of interfacial MnFe{sub 2}O{sub 4} or CoFe{sub 2}O{sub 4}. Instead, the ferrimagnetism is induced by the adjacent Fe{sub 3}O{sub 4} layer and is the result of the stabilization of a spinel phase not achievable in bulk form. Magnetism at the interface region is observable up to 500 K, far beyond the chromite bulk Curie temperature of 50-95 K.

  18. Synchrotron X-ray Absorption and In Vitro Bioactivity of Magnetic Macro/Mesoporous Bioactive Glasses

    Directory of Open Access Journals (Sweden)

    Thanida Charoensuk

    2015-12-01

    Full Text Available Iron oxides in macro/mesoporous bioactive glasses were characterized by synchrotron X-ray absorption near edge structure (XANES spectroscopy. This magnetic phase was introduced by adding Fe(NO33 9H2O during the sol-gel synthesis. The obtained bioactive glass scaffolds exhibited superparamagnetism, in which the magnetization was increased with the increase in the Fe molar ratio from 10 to 20%. The linear combination fits of the XANES spectra indicated that the increase in the Fe molar ratio to 20% enhanced the γ-Fe2O3 formation at the expense of the α- Fe2O3 phase. This variation also promoted the formation of fine-grained bone-like apatites on the surface of the scaffolds in the in vitro test. The apatite growth between three and seven days was confirmed by the changing elemental compositions. However, the highest magnetic proportion led to the distortion of the skeleton walls and the collapse of the porous networks.

  19. High-resolution X-ray spectroscopy of the magnetic Of?p star HD148937

    CERN Document Server

    Naze, Y; Walborn, N R

    2011-01-01

    High-resolution data of the peculiar magnetic massive star HD148937 were obtained with Chandra-HETGS, and are presented here in combination with a re-analysis of the older XMM-RGS data. The lines of the high-Z elements (Mg, Si, S) were found to be unshifted and relatively narrow (FWHM of about 800km/s), i.e. narrower than the O line recorded by RGS, which possibly indicates that the hot plasma is multi-thermal and has several origins. These data further indicate a main plasma temperature of about 0.6keV and a formation of the X-ray emission at about one stellar radius above the photosphere. From the spectral fits and the H-to-He line ratios, the presence of very hot plasma is however confirmed, though with a smaller relative strength than for the prototype magnetic oblique rotator $\\theta^1$\\,Ori\\,C. Both stars thus share many similarities, but HD148937 appears less extreme than $\\theta^1$\\,Ori\\,C despite having also a large magnetic confinement parameter.

  20. X-ray emission from the giant magnetosphere of the magnetic O-type star NGC 1624-2

    CERN Document Server

    Petit, V; Wade, G A; Nazé, Y; Owocki, S P; Sundqvist, J O; ud-Doula, A; Fullerton, A; Leutenegger, M; Gagné, M

    2015-01-01

    We observed NGC 1624-2, the O-type star with the largest known magnetic field Bp~20 kG), in X-rays with the ACIS-S camera onboard the Chandra X-ray Observatory. Our two observations were obtained at the minimum and maximum of the periodic Halpha emission cycle, corresponding to the rotational phases where the magnetic field is the closest to equator-on and pole-on, respectively. With these observations, we aim to characterise the star's magnetosphere via the X-ray emission produced by magnetically confined wind shocks. Our main findings are: (i) The observed spectrum of NGC 1624-2 is hard, similar to the magnetic O-type star Theta 1 Ori C, with only a few photons detected below 0.8 keV. The emergent X-ray flux is 30% lower at the Halpha minimum phase. (ii) Our modelling indicated that this seemingly hard spectrum is in fact a consequence of relatively soft intrinsic emission, similar to other magnetic Of?p stars, combined with a large amount of local absorption (~1-3 x 10^22 cm^-2). This combination is necess...

  1. Note: theoretical study on the gas pressure dependence of x-ray yield in TE(111) cavity based electron cyclotron resonance x-ray source.

    Science.gov (United States)

    Selvakumaran, T S; Sen, Soubhadra; Baskaran, R

    2014-11-01

    Adopting Langevin methodology, a pressure dependent frictional force term which represents the collisional effect is added to the Lorentz equation. The electrons are assumed to be starting from the uniformly distributed co-ordinates on the central plane. The trajectory of each electron is numerically simulated by solving the modified Lorentz equation for a given pressure. The Bremsstrahlung x-ray energy spectrum for each electron crossing the cavity wall boundary is obtained using the Duane-Hunt law. The total x-ray yield is estimated by adding the spectral contribution of each electron. The calculated yields are compared with the experimental results and a good agreement is found.

  2. X-ray magnetic circular dichroism and reflection anisotropy spectroscopy Kerr effect studies of capped magnetic nanowires

    Energy Technology Data Exchange (ETDEWEB)

    Cunniffe, J. P.; McNally, D.E.; Liberati, M.; Arenholz, E.; McGuinness, C.; McGilp, J. F.

    2010-03-02

    Aligned Co wires grown on Pt(997) under ultra-high vacuum conditions have been capped successfully by the epitaxial growth of Au monolayers (ML) at room temperature. The samples were kept under vacuum except when transferring between apparatus or when making some of the measurements. No degradation of the Co wires was detected during the measurements. The magneto-optic response of the system was measured using X-ray magnetic circular dichroism (XMCD) at the Co L{sub 2,3} edge and reflection anisotropy spectroscopy (RAS) at near normal incidence, which is sensitive to the normal component of the out-of-plane magnetization via the Kerr effect (MOKE). Capping the wires significantly impacts their magnetic properties. Comparison of the magneto-optic response of the system at X-ray and optical energies reveals small differences that are attributed to the induced moment in the Pt substrate and Au capping layer not picked up by the element specific XMCD measurements. The sensitivity of RAS-MOKE is sufficient to allow the determination of the easy axis direction of the capped wires to within a few degrees. The results for a 6-atom-wide Co wire sample, capped with 6 ML of Au, are consistent with the capped wires possessing perpendicular magnetization.

  3. Electronic Structure of the ID Conductor K0.3MoO3 studied using resonant inelastic x-ray scattering and soft x-ray emission spectroscopy

    Energy Technology Data Exchange (ETDEWEB)

    Learmonth, T.; Glans, P.-A.; McGuinness, C.; Plucinski, L.; Zhang, Y.; Guo, J.-H.; Greenblatt, M.; Smith, K.E.

    2008-09-24

    The electronic structure of the quasi-one dimensional conductor K{sub 0.3}MoO{sub 3} has been measured using high resolution resonant inelastic x-ray scattering and x-ray absorption spectroscopy. The data is compared to that from the related two dimensional insulator {alpha}-MoO{sub 3}. Scattering features are observed from both oxides that are explained in terms of the band momentum selectivity of the scattering process, allowing a comparison of the scattering data to recent band structure calculations.

  4. X-ray speckle experiments on the persistence and disintegration of magnetic memory

    Science.gov (United States)

    Pierce, Michael Scott

    Beautiful theories based on random microscopic disorder have been developed over the past ten years. My goal was to directly compare these theories with precise experiments. To do so, I first developed and then applied coherent x-ray speckle metrology to a series of thin multilayer perpendicular magnetic materials. To directly observe the effects of disorder, increasing degrees of disorder was deliberately introduced into a series of magnetic films. I used coherent x-rays, produced at the Advanced Light Source at Lawrence Berkeley National Laboratory, to generate highly speckled magnetic scattering patterns. The scattering patterns provided both the ensemble average characteristics of the magnetic domains, but were also directly sensitive to the microscopic magnetic domains. The apparently "random" arrangement of the speckles is due to the exact configuration of the magnetic domains in the sample. In effect, each speckle pattern acts as a unique fingerprint for the magnetic domain configuration. Small changes in the domain structure change the speckles, and comparison of the different speckle patterns provides a quantitative determination of how much the domain structure has changed. My experiments quickly answered one longstanding question: How is the magnetic domain configuration at one point on the major hysteresis loop related to the configurations at the same point on the loop during subsequent cycles? This is called microscopic return point memory (RPM). I found the RPM is partial and imperfect in the disordered samples, and completely absent when the disorder was not present. I also introduced and answered a second important, new question: How are the magnetic domains at one point on the major hysteresis loop related to the domains at the complementary point, the inversion symmetric point on the loop, during the same and during subsequent cycles? This is called microscopic complementary point memory (CPM). I found the CPM is also partial and imperfect in the

  5. Double resonance capacitance spectroscopy (DORCAS): A new experimental technique for assignment of X-ray absorption peaks to surface sites of semiconductor

    CERN Document Server

    Ishii, M

    2003-01-01

    As a new microspectroscopy for semiconductor surface analysis using an X-ray beam, double resonance capacitance spectroscopy (DORCAS) is proposed. For a microscopic X-ray absorption measurement, a local capacitance change owing to X-ray induced emission of localized electrons is detected by a microprobe. The applied bias voltage V sub b dependence of the capacitance also provides information on the surface density of state. The resonance of the Fermi energy with a surface level by V sub b control makes possible the selection of the observable surface site in the X-ray absorption measurements, i.e. site-specific spectroscopy. The double resonance of the surface site selection (V sub b resonance) and the resonant X-ray absorption of the selected site (photon energy h nu resonance) enhances the capacitance signal. The DORCAS measurement of the GaAs surface shows correlation peaks at h nu=10.402 keV and V sub b =-0.4 V and h nu=10.429 keV and V sub b =+0.1 V, indicating that these resonant X-ray absorption peaks ...

  6. Effect of Coulomb interaction on the X-ray magnetic circular dichroism spin sum rule in rare earths

    NARCIS (Netherlands)

    Teramura, Y; Tanaka, A; Thole, BT; Jo, T

    A deviation from the spin sum rule, which relates the integrated intensity of the X-ray magnetic circular dichroism (MCD) signal to the expectation value of the spin operator S-z ((S-z)), is numerically calculated in the case of the 3d --> 4f absorption for rare earths from the trivalent Ce to Tm.

  7. X-ray magnetic circular dichroism spectra and distortions at Fe2+ L(2,3) edges

    NARCIS (Netherlands)

    Wang, X.; de Groot, F.M.F.; Cramer, S.P.

    1996-01-01

    We have shown from ligand field multiplet calculations that the shape of X-ray magnetic circular dichroism (XMCD) spectra changes drastically with the distortion parameter Ds. The temperature dependence study of XMCD makes it possible to determine both Ds and spin-orbit coupling.

  8. X-ray magnetic circular dichroism spectra and distortions at Fe2+ L(2,3) edges

    NARCIS (Netherlands)

    Wang, X.; de Groot, F.M.F.; Cramer, S.P.

    We have shown from ligand field multiplet calculations that the shape of X-ray magnetic circular dichroism (XMCD) spectra changes drastically with the distortion parameter Ds. The temperature dependence study of XMCD makes it possible to determine both Ds and spin-orbit coupling.

  9. A Novel Method for Studying Thermal Motion and Point Defects in Crystals by X-Ray Resonant Diffraction

    Science.gov (United States)

    Dmitrienko, V. E.; Ishida, K.; Kirfel, A.; Kokubun, J.; Ovchinnikova, E. N.

    2003-01-01

    After an introductory survey of the X-ray resonant anisotropy, we present a novel X-ray method to observe thermal-motion-induced (TMI) and point-defect-induced (PDI) distortions of electronic states of atoms. This method uses the idea that, in general, the local atomic environment becomes less symmetric owing to point defects and/or the thermal vibrations of the atoms in a crystal. As a result of this phenomenon, an additional anisotropy of the resonant scattering factors can occur and "forbidden" Bragg reflections can be excited near the absorption edges. Examples of crystals are discussed (Ge, Y3Fe5O12) where TMI and PDI reflections can be found. The tensor structure factors of the both types of reflections are calculated. According to our theory, the TMI reflection structure factors are proportional to the vibration correlations, u∥2 and u⊥2, of neighboring atoms, and it is inferred that u∥2 provides the main contribution to the thermal-motion-induced anisotropy of X-ray resonant scattering. The TMI reflections in Ge were recently observed by Kokubun et al. (Phys. Rev. B64, 073203 (2001)), Kirfel et al. (in press), and Colella et al. (in press) in accordance with our prediction. For the 006 reflection, the intensity increases about 25 times with the temperature increasing from 30 to 735 K. Owing to their resonant character, the PDI reflections allow to separately study both impurity atoms and host atoms of different types. The considered phenomena can provide a very sensitive method for studying point defects because only the atoms that are affected by defects contribute to the PDI reflections.

  10. X-ray absorption and resonant inelastic x-ray scattering (RIXS) show the presence of Cr{sup +} at the surface and in the bulk of CrF{sub 2}

    Energy Technology Data Exchange (ETDEWEB)

    Jiménez-Mier, J. [Instituto de Ciencias Nucleares, UNAM, 04510 México DF, México (Mexico); Olalde-Velasco, P. [The Advanced Light Source, Lawrence Berkeley Laboratory, Berkeley, CA 94720 (United States); Swiss Light Source. Paul Scherrer Institut, CH-5232 Villigen PSI (Switzerland); Yang, W.-L.; Denlinger, J. [The Advanced Light Source, Lawrence Berkeley Laboratory, Berkeley, CA 94720 (United States)

    2015-07-23

    X-Ray absorption and resonant inelastic x-ray scattering (RIXS) spectra of CrF{sub 2} recorded at the chromium L{sub 2,3} are presented. An atomic multiplet crystal field calculation is compared with the experimental data. Experiment and theory are in agreement once the calculation includes three chromium oxidation states, namely Cr{sup +}, Cr{sup 2+}, and Cr{sup 3+}. X-Ray absorption allows a direct determination of the surface oxidation, while the RIXS spectra shows the presence of these three oxidation states in the sample bulk. To give a quantitative interpretation of the RIXS data the effect of the incomming and outgoing photon penetration depth and self-absorption must be considered. For the much simpler case of MnF{sub 2}, with only one metal oxidation state, the measured RIXS spectra relative intensities are found to be proportional to the square of the sample attenuation length.

  11. Development of an alternating magnetic-field-assisted finishing process for microelectromechanical systems micropore x-ray optics.

    Science.gov (United States)

    Riveros, Raul E; Yamaguchi, Hitomi; Mitsuishi, Ikuyuki; Takagi, Utako; Ezoe, Yuichiro; Kato, Fumiki; Sugiyama, Susumu; Yamasaki, Noriko; Mitsuda, Kazuhisa

    2010-06-20

    X-ray astronomy research is often limited by the size, weight, complexity, and cost of functioning x-ray optics. Micropore optics promises an economical alternative to traditional (e.g., glass or foil) x-ray optics; however, many manufacturing difficulties prevent micropore optics from being a viable solution. Ezoe et al. introduced microelectromechanical systems (MEMS) micropore optics having curvilinear micropores in 2008. Made by either deep reactive ion etching or x-ray lithography, electroforming, and molding (LIGA), MEMS micropore optics suffer from high micropore sidewall roughness (10-30nmrms) which, by current standards, cannot be improved. In this research, a new alternating magnetic-field-assisted finishing process was developed using a mixture of ferrofluid and microscale abrasive slurry. A machine was built, and a set of working process parameters including alternating frequency, abrasive size, and polishing time was selected. A polishing experiment on a LIGA-fabricated MEMS micropore optic was performed, and a change in micropore sidewall roughness of 9.3+/-2.5nmrms to 5.7+/-0.7nmrms was measured. An improvement in x-ray reflectance was also seen. This research shows the feasibility and confirms the effects of this new polishing process on MEMS micropore optics.

  12. Crystallographic origin of perpendicular magnetic anisotropy in CoPt film: polarized x-ray absorption study

    Energy Technology Data Exchange (ETDEWEB)

    Pandey, K [National University of Singapore; Chen, J [National University of Singapore; Liu, T [Oak Ridge National Laboratory (ORNL); Sun, C [Singapore Synchrotron Light Source; Chow, G [National University of Singapore

    2009-01-01

    Crystallographic structure, growth induced miscibility gap and strain in Ta/Co100 xPtx (0 x 43 at%)/Ru/Ta/glass films deposited at ambient temperature were investigated using polarized x-ray absorption spectroscopy to clarify the origin of observed perpendicular magnetic anisotropy (PMA) in Co72Pt28 film. Extended x-ray absorption fine structure spectroscopy data at Co K-edge showed that Co has a similar local atomic environment and averaged interatomic distance in the in-plane and out-of-plane polarization geometries for Co72Pt28, ruling out the contribution of magneto-elastic anisotropy and growth induced structural anisotropy as the origin of PMA. A large PMA in Co72Pt28 film was attributed to the preferred hexagonal close-packed stacking as observed using the x-ray absorption near-edge structure spectroscopy.

  13. Directly Characterizing the Relative Strength and Momentum Dependence of Electron-Phonon Coupling Using Resonant Inelastic X-Ray Scattering

    Science.gov (United States)

    Devereaux, T. P.; Shvaika, A. M.; Wu, K.; Wohlfeld, K.; Jia, C. J.; Wang, Y.; Moritz, B.; Chaix, L.; Lee, W.-S.; Shen, Z.-X.; Ghiringhelli, G.; Braicovich, L.

    2016-10-01

    The coupling between lattice and charge degrees of freedom in condensed matter materials is ubiquitous and can often result in interesting properties and ordered phases, including conventional superconductivity, charge-density wave order, and metal-insulator transitions. Angle-resolved photoemission spectroscopy and both neutron and nonresonant x-ray scattering serve as effective probes for determining the behavior of appropriate, individual degrees of freedom—the electronic structure and lattice excitation, or phonon dispersion, respectively. However, each provides less direct information about the mutual coupling between the degrees of freedom, usually through self-energy effects, which tend to renormalize and broaden spectral features precisely where the coupling is strong, impacting one's ability to quantitatively characterize the coupling. Here, we demonstrate that resonant inelastic x-ray scattering, or RIXS, can be an effective tool to directly determine the relative strength and momentum dependence of the electron-phonon coupling in condensed matter systems. Using a diagrammatic approach for an eight-band model of copper oxides, we study the contributions from the lowest-order diagrams to the full RIXS intensity for a realistic scattering geometry, accounting for matrix element effects in the scattering cross section, as well as the momentum dependence of the electron-phonon coupling vertex. A detailed examination of these maps offers a unique perspective into the characteristics of electron-phonon coupling, which complements both neutron and nonresonant x-ray scattering, as well as Raman and infrared conductivity.

  14. Directly Characterizing the Relative Strength and Momentum Dependence of Electron-Phonon Coupling Using Resonant Inelastic X-Ray Scattering

    Energy Technology Data Exchange (ETDEWEB)

    Devereaux, T.P.; Shvaika, A.M.; Wu, K.; Wohlfeld, K.; Jia, C.J.; Wang, Y.; Moritz, B.; Chaix, L.; Lee, W.-S.; Shen, Z.-X.; Ghiringhelli, G.; Braicovich, L.

    2016-10-25

    The coupling between lattice and charge degrees of freedom in condensed matter materials is ubiquitous and can often result in interesting properties and ordered phases, including conventional superconductivity, charge-density wave order, and metal-insulator transitions. Angle-resolved photoemission spectroscopy and both neutron and nonresonant x-ray scattering serve as effective probes for determining the behavior of appropriate, individual degrees of freedom—the electronic structure and lattice excitation, or phonon dispersion, respectively. However, each provides less direct information about the mutual coupling between the degrees of freedom, usually through self-energy effects, which tend to renormalize and broaden spectral features precisely where the coupling is strong, impacting one’s ability to quantitatively characterize the coupling. Here, we demonstrate that resonant inelastic x-ray scattering, or RIXS, can be an effective tool to directly determine the relative strength and momentum dependence of the electron-phonon coupling in condensed matter systems. Using a diagrammatic approach for an eight-band model of copper oxides, we study the contributions from the lowest-order diagrams to the full RIXS intensity for a realistic scattering geometry, accounting for matrix element effects in the scattering cross section, as well as the momentum dependence of the electron-phonon coupling vertex. A detailed examination of these maps offers a unique perspective into the characteristics of electron-phonon coupling, which complements both neutron and nonresonant x-ray scattering, as well as Raman and infrared conductivity.

  15. Direct evidence of Ni magnetic moment in TbNi{sub 2}Mn—X-ray magnetic circular dichroism

    Energy Technology Data Exchange (ETDEWEB)

    Yu, D.H., E-mail: dyu@ansto.gov.au [Bragg Institute, Australian Nuclear Science and Technology Organisation, Lucas Heights, Sydney, NSW 2234 (Australia); Huang, Meng-Jie [National Synchrotron Radiation Research Center, 101 Hsin-Ann Road, Hsinchu Science Park, Hsinchu 30076, Taiwan (China); Wang, J.L. [Bragg Institute, Australian Nuclear Science and Technology Organisation, Lucas Heights, Sydney, NSW 2234 (Australia); School of Physical, Environmental and Mathematical Sciences, University of New South Wales, Canberra at the Australian Defense Force Academy, Sydney, ACT 2600 (Australia); Institute for Superconductivity and Electronic Materials, University of Wollongong, Wollongong, NSW 2522 (Australia); Su, Hui-Chia; Lin, Hong-Ji; Chen, Chien-Te [National Synchrotron Radiation Research Center, 101 Hsin-Ann Road, Hsinchu Science Park, Hsinchu 30076, Taiwan (China); Campbell, S.J. [School of Physical, Environmental and Mathematical Sciences, University of New South Wales, Canberra at the Australian Defense Force Academy, Sydney, ACT 2600 (Australia)

    2014-12-15

    We have investigated the individual magnetic moments of Ni, Mn and Tb atoms in the intermetallic compound TbNi{sub 2}Mn in the Laves phase (magnetic phase transition temperature T{sub C} ∼131 K) by X-ray magnetic circular dichroism (XMCD) studies at 300 K, 80 K and 20 K. Analyses of the experimental results reveal that Ni atoms at 20 K in an applied magnetic field of 1 T carry an intrinsic magnetic moment of spin and orbital magnetic moment contributions 0.53±0.01 μ{sub B} and 0.05±0.01 μ{sub B}, respectively. These moment values are similar to those of the maximum saturated moment of Ni element. A very small magnetic moment of order <0.1 μ{sub B} has been measured for Mn. This suggests that Mn is antiferromagnetically ordered across the two nearly equally occupied sites of 16d and 8a. A magnetic moment of up to ∼0.3 μ{sub B} has been observed for the Tb atoms. Identification of a magnetic moment on the Ni atoms has provided further evidence for the mechanism of enhancement of the magnetic phase transition temperature in TbNi{sub 2}Mn compared with TbNi{sub 2} (T{sub C}∼37.5 K) and TbMn{sub 2} (T{sub C}∼54 K) due to rare earth–transition metal (R–T) and transition metal–transition metal (T–T) interactions. The behaviour of the X-ray magnetic circular dichroism spectra of TbNi{sub 2}Mn at 300 K, 80 K and 20 K – above and below the magnetic ordering temperature T{sub C} ∼131 K – is discussed. - Highlights: • We study the magnetic moment of TbNi{sub 2}Mn with XMCD. • We observe directly the Ni intrinsic magnetic moment in TbNi{sub 2}Mn. • We find that Mn ordered antiferromagnetically across the 16d and 8a sites. • We confirm the mechanism for increasing the magnetic phase transition temperature.

  16. Collimating Montel mirror as part of a multi-crystal analyzer system for resonant inelastic X-ray scattering.

    Science.gov (United States)

    Kim, Jungho; Shi, Xianbo; Casa, Diego; Qian, Jun; Huang, XianRong; Gog, Thomas

    2016-07-01

    Advances in resonant inelastic X-ray scattering (RIXS) have come in lockstep with improvements in energy resolution. Currently, the best energy resolution at the Ir L3-edge stands at ∼25 meV, which is achieved using a diced Si(844) spherical crystal analyzer. However, spherical analyzers are limited by their intrinsic reflection width. A novel analyzer system using multiple flat crystals provides a promising way to overcome this limitation. For the present design, an energy resolution at or below 10 meV was selected. Recognizing that the angular acceptance of flat crystals is severely limited, a collimating element is essential to achieve the necessary solid-angle acceptance. For this purpose, a laterally graded, parabolic, multilayer Montel mirror was designed for use at the Ir L3-absorption edge. It provides an acceptance larger than 10 mrad, collimating the reflected X-ray beam to smaller than 100 µrad, in both vertical and horizontal directions. The performance of this mirror was studied at beamline 27-ID at the Advanced Photon Source. X-rays from a diamond (111) monochromator illuminated a scattering source of diameter 5 µm, generating an incident beam on the mirror with a well determined divergence of 40 mrad. A flat Si(111) crystal after the mirror served as the divergence analyzer. From X-ray measurements, ray-tracing simulations and optical metrology results, it was established that the Montel mirror satisfied the specifications of angular acceptance and collimation quality necessary for a high-resolution RIXS multi-crystal analyzer system.

  17. 4f orbital and spin magnetism in cerium intermetallic compounds studied by magnetic circular x-ray dichroism

    Science.gov (United States)

    Schillé, J. Ph.; Bertran, F.; Finazzi, M.; Brouder, Ch.; Kappler, J. P.; Krill, G.

    1994-08-01

    Magnetic circular x-ray dichroism experiments at the M4,5 absorption edges of cerium in the intermetallic compounds CeCuSi, CeRh3B2, and CeFe2 are reported. By applying general sum rules, it is shown that these experiments are able to yield both the magnitude and the direction of the 4f magnetic moment on Ce. An estimation of the orbital contribution to those 4f moments is given. Our experiments demonstrate the existence of a 4f magnetic moment on Ce in CeFe2 and confirm the extreme sensitivity of the 4f orbital contribution to the degree of localization of the 4f electrons. This 4f orbital contribution is significantly higher than the one predicted from spin-resolved band-structure calculations.

  18. A portable high-field pulsed-magnet system for single-crystal x-ray scattering studies.

    Science.gov (United States)

    Islam, Zahirul; Ruff, Jacob P C; Nojiri, Hiroyuki; Matsuda, Yasuhiro H; Ross, Kathryn A; Gaulin, Bruce D; Qu, Zhe; Lang, Jonathan C

    2009-11-01

    We present a portable pulsed-magnet system for x-ray studies of materials in high magnetic fields (up to 30 T). The apparatus consists of a split-pair of minicoils cooled on a closed-cycle cryostat, which is used for x-ray diffraction studies with applied field normal to the scattering plane. A second independent closed-cycle cryostat is used for cooling the sample to near liquid helium temperatures. Pulsed magnetic fields (approximately 1 ms in total duration) are generated by discharging a configurable capacitor bank into the magnet coils. Time-resolved scattering data are collected using a combination of a fast single-photon counting detector, a multichannel scaler, and a high-resolution digital storage oscilloscope. The capabilities of this instrument are used to study a geometrically frustrated system revealing strong magnetostrictive effects in the spin-liquid state.

  19. Voltage-controlled magnetic anisotropy in Fe|MgO tunnel junctions studied by x-ray absorption spectroscopy

    Energy Technology Data Exchange (ETDEWEB)

    Miwa, Shinji, E-mail: miwa@mp.es.osaka-u.ac.jp; Matsuda, Kensho; Tanaka, Kazuhito; Goto, Minori; Suzuki, Yoshishige [Graduate School of Engineering Science, Osaka University, Toyonaka, Osaka 560-8531 (Japan); Kotani, Yoshinori; Nakamura, Tetsuya [Japan Synchrotron Radiation Research Institute/SPring-8, Sayo, Hyogo 679-5198 (Japan)

    2015-10-19

    In this study, voltage-controlled magnetic anisotropy (VCMA) in Fe|MgO tunnel junctions was investigated via the magneto-optical Kerr effect, soft x-ray absorption spectroscopy, and magnetic circular dichroism spectroscopy. The Fe|MgO tunnel junctions showed enhanced perpendicular magnetic anisotropy under external negative voltage, which induced charge depletion at the Fe|MgO interface. Despite the application of voltages of opposite polarity, no trace of chemical reaction such as a redox reaction attributed to O{sup 2−} migration was detected in the x-ray absorption spectra of the Fe. The VCMA reported in the Fe|MgO-based magnetic tunnel junctions must therefore originate from phenomena associated with the purely electric effect, that is, surface electron doping and/or redistribution induced by an external electric field.

  20. MRI (Magnetic Resonance Imaging)

    Science.gov (United States)

    ... and Procedures Medical Imaging MRI (Magnetic Resonance Imaging) MRI (Magnetic Resonance Imaging) Share Tweet Linkedin Pin it More sharing options ... usually given through an IV in the arm. MRI Research Programs at FDA Magnetic Resonance Imaging (MRI) ...

  1. X-ray scattering and magnetic susceptibility study of doped CuGeO sub 3

    CERN Document Server

    Wang, Y J; Lamarra, S C; Chou, F C; Kim, Y J; Masuda, T; Tsukada, I; Uchinokura, K; Birgeneau, R J

    2003-01-01

    We report comprehensive synchrotron x-ray scattering and magnetic susceptibility studies of the doped spin-Peierls materials Cu sub 1 sub - sub x Zn sub x GeO sub 3 and CuGe sub 1 sub - sub y Si sub y O sub 3. Temperature versus dopant concentration phase diagrams are mapped out for both Zn and Si dopants. The phase diagrams of both Cu sub 1 sub - sub x Zn sub x GeO sub 3 and CuGe sub 1 sub - sub y Si sub y O sub 3 closely resemble that of Cu sub 1 sub - sub x Mg sub x GeO sub 3 , including the observation that the spin gap is established at a much higher temperature than the temperature at which the spin-Peierls dimerization attains long-range order. The spin-Peierls transitions in doped samples exhibit unusual phase transition behavior, characterized by highly rounded phase transitions, Lorentzian squared lineshapes, and very long relaxation times. Phenomenological explanations for these observations are given by considering the effects of competing random bond interactions as well as random fields generate...

  2. X-ray and Rotational Luminosity Correlation and Magnetic Heating of the Radio Pulsars

    CERN Document Server

    Shibata, S; Yatsu, Y; Enoto, T; Bamba, A

    2016-01-01

    Previous works have suggested a correlation between the X-ray luminosity Lx and the rotational luminosity Lrot of the radio pulsars.However, none of the obtained regression lines are statistically acceptable due to large scatters. We construct a statistical model which has an intrinsic Lx-Lrot relation and reproduces the observed Lx distribution about it by using a Monte Carlo simulator, which takes into account the effects obscuring the intrinsic relation,i.e., the anisotropy of radiation, additional heating, uncertainty in distance and detection limit of the instruments. From the ATNF pulsar catalog we collect 57 `ordinary radio pulsars' with significant detection and 42 with upper limits.The sample does not include the high-magnetic field pulsars (>10^{13} G), which are separately analyzed. We obtain a statistically acceptable relation Lx (0.5 - 10 keV)= 10^{31.69} (Lrot / L_0)^{c_1} with c_1 = 1.03 \\pm 0.27 and L_0 =10^{35.38}. The distribution about the obtained Lx-Lrot relation is reproduced well by the...

  3. X-rays From Magnetic Flares In Cygnus X-1 The Role Of A Transition Layer

    CERN Document Server

    Nayakshin, S; Nayakshin, Sergei; Dove, James B.

    1998-01-01

    The spectrum of Seyfert 1 Galaxies is very similar to that of several Galactic Black Hole Candidates (GBHCs) in their hard state, suggestive that both classes of objects have similar physical processes. While it appears that an accretion disk corona (ADC) model, where the corona sandwiches the cold accretion disk, is capable of explaining the observations of Seyfert galaxies, recent work has shown that this model is problematic for GBHCs. To address the differences in the spectra of Seyferts and GBHCs, we consider the structure of the atmosphere of the accretion disk in a region near an active magnetic flare (we refer to this region as transition layer). We show that the transition layer is subject to a thermal instability. Due to the much higher ionizing X-ray flux in GBHCs, the only stable solution for the upper layer of the accretion disk is that in which it is highly ionized and is at the Compton temperature ($kT \\sim $ a few keV). Using numerical simulations for a slab geometry ADC, we show that the pres...

  4. Resonant inelastic X-ray spectroscopy of atoms and simple molecules: Satellite features and dependence on energy detuning and photon polarization

    Energy Technology Data Exchange (ETDEWEB)

    Žitnik, M., E-mail: matjaz.zitnik@ijs.si [Jožef Stefan Institute, P.O. Box 3000, SI-1001 Ljubljana (Slovenia); University of Ljubljana, Faculty of Mathematics and Physics, Jadranska 21, SI-1000 Ljubljana (Slovenia); Kavčič, M.; Bohinc, R.; Bučar, K.; Mihelič, A. [Jožef Stefan Institute, P.O. Box 3000, SI-1001 Ljubljana (Slovenia); Cao, W. [Research Centre for Molecular Materials, University of Oulu, P.O. Box 3000, FIN-90014 Oulu (Finland); Guillemin, R.; Journel, L.; Marchenko, T.; Carniato, S.; Kawerk, E. [Sorbonne Universités, UPMC Univ Paris 06, UMR 7614, Laboratoire de Chimie Physique Matière et Rayonnement, F-75005 Paris (France); CNRS, UMR 7614, Laboratoire de Chimie Physique Matière et Rayonnement, F-75005 Paris (France); Piancastelli, M.N. [Sorbonne Universités, UPMC Univ Paris 06, UMR 7614, Laboratoire de Chimie Physique Matière et Rayonnement, F-75005 Paris (France); CNRS, UMR 7614, Laboratoire de Chimie Physique Matière et Rayonnement, F-75005 Paris (France); Department of Physics and Astronomy, Uppsala University, P.O. Box 516, 75120 Uppsala (Sweden); Simon, M. [Sorbonne Universités, UPMC Univ Paris 06, UMR 7614, Laboratoire de Chimie Physique Matière et Rayonnement, F-75005 Paris (France); CNRS, UMR 7614, Laboratoire de Chimie Physique Matière et Rayonnement, F-75005 Paris (France)

    2015-10-15

    We summarize recent results dealing with high resolution (resonant) X-ray spectroscopy of atomic and molecular targets in the tender X-ray energy region. We comment on advantages, new possibilities and problems related to RIXS spectroscopy with respect to the standard photoabsorption technique, where scanning the probe energy is the only option. In particular, three research areas are covered: X-ray emission mediated by energy dependent photoabsorption to multi-electron excited states, the Cl K core-hole clock studies exemplified by systematic study of chloro(fluoro)-hydrocarbon targets and the polarization dependent X-ray emission studies. Due to its spectral selectivity and simultaneous detection capability, high resolution wavelength dispersive X-ray spectroscopy has the capability to resolve structural and dynamical properties of matter within new instrumentation frontiers.

  5. Absorption lines from magnetically driven winds in X-ray binaries

    Science.gov (United States)

    Chakravorty, S.; Petrucci, P.-O.; Ferreira, J.; Henri, G.; Belmont, R.; Clavel, M.; Corbel, S.; Rodriguez, J.; Coriat, M.; Drappeau, S.; Malzac, J.

    2016-05-01

    Context. High resolution X-ray spectra of black hole X-ray binaries (BHBs) show blueshifted absorption lines suggesting the presence of outflowing winds. Furthermore, observations show that the disk winds are equatorial and they occur in the Softer (disk dominated) states of the outburst and are less prominent or absent in the Harder (power-law dominated) states. Aims: We want to test whether the self-similar magneto-hydrodynamic (MHD) accretion-ejection models can explain the observational results for accretion disk winds in BHBs. In our models, the density at the base of the outflow from the accretion disk is not a free parameter. This mass loading is determined by solving the full set of dynamical MHD equations without neglecting any physical term. Thus, the physical properties of the outflow depend on and are controlled by the global structure of the disk. Methods: We studied different MHD solutions characterized by different values of the disk aspect ratio (ɛ) and the ejection efficiency (p). We also generate two kinds of MHD solutions depending on the absence (cold solution) or presence (warm solution) of heating at the disk surface. Such heating could be either from dissipation of energy due to MHD turbulence in the disk or from illumination of the disk surface. Warm solutions can have large (>0.1) values of p, which would imply larger wind mass loading at the base of the outflow. We use each of these MHD solutions to predict the physical parameters (distance, density, velocity, magnetic field, etc.) of an outflow. Motivated by observational results, we have put limits on the ionization parameter (ξ), column density, and timescales. Further constraints were derived for the allowed values of ξ from thermodynamic instability considerations, particularly for the Hard SED. These physical constraints were imposed on each of these outflows to select regions within it, which are consistent with the observed winds. Results: The cold MHD solutions are found to be

  6. A new soft X-ray magnetic circular dichroism facility at the BSRF beamline 4B7B

    Science.gov (United States)

    Guo, Zhi-Ying; Hong, Cai-Hao; Xing, Hai-Ying; Tang, Kun; Zheng, Lei; Xui, Wei; Chen, Dong-Liang; Cui, Ming-Qi; Zhao, Yi-Dong

    2015-04-01

    X-ray magnetic circular dichroism (XMCD) has become an important and powerful tool because it allows the study of material properties in combination with elemental specificity, chemical state specificity, and magnetic specificity. A new soft X-ray magnetic circular dichroism apparatus has been developed at the Beijing Synchrotron Radiation Facility (BSRF). The apparatus combines three experimental conditions: an ultra-high-vacuum environment, moderate magnetic fields and in-situ sample preparation to measure the absorption signal. We designed a C-type dipole electromagnet that provides magnetic fields up to 0.5 T in parallel (or anti-parallel) direction relative to the incoming X-ray beam. The performances of the electromagnet are measured and the results show good agreement with the simulation ones. Following film grown in situ by evaporation methods, XMCD measurements are performed. Combined polarization corrections, the magnetic moments of the Fe and Co films determined by sum rules are consistent with other theoretical predictions and experimental measurements. Supported by National Natural Science Foundation of China (61204008)

  7. Burn Out or Fade Away? On the X-ray and Magnetic Death of Intermediate Mass Stars

    CERN Document Server

    Drake, Jeremy J; Kashyap, Vinay; Guenther, H Moritz; Wright, Nicholas J

    2014-01-01

    The nature of the mechanisms apparently driving X-rays from intermediate mass stars lacking strong convection zones or massive winds remains poorly understood, and the possible role of hidden, lower mass close companions is still unclear. A 20ks Chandra HRC-I observation of HR 4796A, an 8 Myr old main sequence A0 star devoid of close stellar companions, has been used to search for a signature or remnant of magnetic activity from the Herbig Ae phase. X-rays were not detected and the X-ray luminosity upper limit was L_X =< 1.3x10^27 erg/s. The result is discussed in the context of various scenarios for generating magnetic activity, including rotational shear and subsurface convection. A dynamo driven by natal differential rotation is unlikely to produce observable X rays, chiefly because of the difficulty in getting the dissipated energy up to the surface of the star. A subsurface convection layer produced by the ionisation of helium could host a dynamo that should be effective throughout the main-sequence b...

  8. The X-ray properties of the magnetic Cataclysmic Variable UU Col

    CERN Document Server

    De Martino, D; Mukai, K; Bonnet-Bidaud, J M; Burwitz, V; Gänsicke, B T; Haberl, F; Mouchet, M

    2006-01-01

    XMM-Newton observations aimed at determining for the first time the broad-band X-ray properties of the faint high galactic latitude Intermediate Polar UU Col are presented. We performed X-ray timing analysis in different energy ranges of the EPIC cameras which reveals the dominance of the 863s white dwarf rotational period. The spin pulse is strongly energy dependent. Weak variabilities at the beat 935s and at the 3.5hr orbital periods are also observed, but the orbital modulation is detected only below 0.5keV. Simultaneous UV and optical photometry shows that the spin pulse is anti-phased with respect to the hard X-rays. Analysis of the EPIC and RGS spectra reveals the complexity of the X-ray emission, being composed of a soft 50eV black--body component and two optically thin emission components at 0.2keV and 11keV strongly absorbed by dense material with an equivalent hydrogen column density of 10**(23)cm**(-2) partially (50%) covering the X-ray source. The complex X-ray and UV/optical temporal behaviour in...

  9. High-Resolution X-ray Emission and X-ray Absorption Spectroscopy

    NARCIS (Netherlands)

    Groot, F.M.F. de

    2000-01-01

    In this review, high-resolution X-ray emission and X-ray absorption spectroscopy will be discussed. The focus is on the 3d transition-metal systems. To understand high-resolution X-ray emission and reso-nant X-ray emission, it is first necessary to spend some time discussing the X-ray absorption

  10. Resonant soft X-ray emission spectroscopy of vanadium oxides andrelated compounds

    Energy Technology Data Exchange (ETDEWEB)

    Schmitt, Thorsten

    2004-11-01

    areas showed homogeneous distribution of Mn substituting for Zn a 2{sup +} state in the ZnO lattice. Ferromagnetic Resonance (FMR) technique is used to confirm the existence of ferromagnetic ordering at temperatures as high as 425K. The ab initio calculations were found to be consistent with the observation of ferromagnetism arising from fully polarized Mn 2{sup +} state. The key to observed room temperature ferromagnetism in this system is the low temperature processing, which prevents formation of clusters, secondary phases and the host ZnO from becoming n-type. The electronic structure of the same Mn doped ZnO thin films studied using XAS, XES and RIXS. revealed a strong hybridization between Mn 3d and O 2p states, which is an important characteristic of a Dilute magnetic Semiconductor (DMS). It is shown that the various processing conditions like sintering temperature, dopant concentration and the properties of precursors used for making of DMS have a great influence on the final properties. Use of various experimental techniques to verify the physical properties, and to understand the mechanism involved to give rise to ferromagnetism is presented. Methods to improve the magnetic moment in Mn doped ZnO are also described. New promising DMS materials (such as Cu doped ZnO are explored). The demonstrated new capability to fabricate powder, pellets, and thin films of room temperature ferromagnetic semiconductors thus makes possible the realization of a wide range of complex elements for a variety of new multifunctional phenomena related to Spintronic devices as well as magneto-optic components.

  11. Resonant soft X-ray emission spectroscopy of vanadium oxides andrelated compounds

    Energy Technology Data Exchange (ETDEWEB)

    Schmitt, Thorsten [Uppsala Univ. (Sweden)

    2004-01-01

    areas showed homogeneous distribution of Mn substituting for Zn a 2+ state in the ZnO lattice. Ferromagnetic Resonance (FMR) technique is used to confirm the existence of ferromagnetic ordering at temperatures as high as 425K. The ab initio calculations were found to be consistent with the observation of ferromagnetism arising from fully polarized Mn 2+ state. The key to observed room temperature ferromagnetism in this system is the low temperature processing, which prevents formation of clusters, secondary phases and the host ZnO from becoming n-type. The electronic structure of the same Mn doped ZnO thin films studied using XAS, XES and RIXS. revealed a strong hybridization between Mn 3d and O 2p states, which is an important characteristic of a Dilute magnetic Semiconductor (DMS). It is shown that the various processing conditions like sintering temperature, dopant concentration and the properties of precursors used for making of DMS have a great influence on the final properties. Use of various experimental techniques to verify the physical properties, and to understand the mechanism involved to give rise to ferromagnetism is presented. Methods to improve the magnetic moment in Mn doped ZnO are also described. New promising DMS materials (such as Cu doped ZnO are explored). The demonstrated new capability to fabricate powder, pellets, and thin films of room temperature ferromagnetic semiconductors thus makes possible the realization of a wide range of complex elements for a variety of new multifunctional phenomena related to Spintronic devices as well as magneto-optic components.

  12. A full-field transmission x-ray microscope for time-resolved imaging of magnetic nanostructures

    Energy Technology Data Exchange (ETDEWEB)

    Ewald, J.; Nisius, T.; Abbati, G.; Baumbach, S.; Overbuschmann, J.; Wilhein, T. [Institute for X-Optics (IXO), Hochschule Koblenz, Joseph-Rovan-Allee 2, 53424 Remagen (Germany); Wessels, P.; Wieland, M.; Drescher, M. [The Hamburg Centre for Ultrafast Imaging (CUI), University of Hamburg, Luruper Chaussee 149, 22761 Hamburg (Germany); Institut für Experimentalphysik, University of Hamburg, Luruper Chaussee 149, 22761 Hamburg (Germany); Vogel, A. [Institut für Angewandte Physik, University of Hamburg, Jungiusstraße 11, 20355 Hamburg (Germany); Viefhaus, J. [Deutsches Elektronen-Synchrotron (DESY), Notkestraße 85, 22607 Hamburg (Germany); Meier, G. [The Hamburg Centre for Ultrafast Imaging (CUI), University of Hamburg, Luruper Chaussee 149, 22761 Hamburg (Germany); Max Planck Institute for the Structure and Dynamics of Matter, Luruper Chaussee 149, 22761 Hamburg (Germany)

    2016-01-28

    Sub-nanosecond magnetization dynamics of small permalloy (Ni{sub 80}Fe{sub 20}) elements has been investigated with a new full-field transmission microscope at the soft X-ray beamline P04 of the high brilliance synchrotron radiation source PETRA III. The soft X-ray microscope generates a flat-top illumination field of 20 μm diameter using a grating condenser. A tilted nanostructured magnetic sample can be excited by a picosecond electric current pulse via a coplanar waveguide. The transmitted light of the sample plane is directly imaged by a micro zone plate with < 65 nm resolution onto a 2D gateable X-ray detector to select one particular bunch in the storage ring that probes the time evolution of the dynamic information successively via XMCD spectromicroscopy in a pump-probe scheme. In the experiments it was possible to generate a homogeneously magnetized state in patterned magnetic layers by a strong magnetic Oersted field pulse of 200 ps duration and directly observe the recovery to the initial flux-closure vortex patterns.

  13. First results of the resonant inelastic X-ray scattering station at the ADRESS beamline at the Swiss Light Source

    Energy Technology Data Exchange (ETDEWEB)

    Schmitt, Thorsten; Strocov, Vladimir; Schlappa, Justina; Patthey, Luc [Swiss Light Source, Paul Scherrer Institut, CH-5232 Villigen PSI (Switzerland); Ghiringhelli, Giacomo; Piazzalunga, Andrea; Dallera, Claudia; Braicovich, Lucio [Politecnico di Milano (Italy); Wang, Xiaoqiang; Grioni, Marco [EPFL Lausanne (Switzerland)

    2008-07-01

    Resonant inelastic X-ray scattering (RIXS) is a powerful bulk-sensitive probe of the electronic structure of condensed matter with atomic and orbital sensitivity. It is an unique tool for determining the energy and symmetry of charge neutral electronic excitations (e.g. crystal field or spin-flip excitations) in strongly correlated materials. The ADvanced RESonant Spectroscopies (ADRESS) beamline at the Swiss Light Source (SLS) features advanced instrumentation for RIXS. This year it will be complemented by instrumentation for Angle-Resolved Photoelectron Spectroscopy. The RIXS station is equipped with a spectrometer (resolving power {approx}12000 for 1 keV) so-called SAXES (Super Advanced X-ray Emission Spectrograph) based on a variable line spacing spherical grating. The RIXS station is open since spring 2007 and was undergoing the operation tests during the 2nd half of 2007. We report on first results obtained with RIXS on transition metal monoxides (NiO, MnO and CuO) as reference compounds. These results demonstrate the capability of this set-up for RIXS studies on strongly correlated materials with unprecedented ultra-high resolution.

  14. 核磁共振、X射线小角散射以及计算机模拟相结合构建生物大分子复合物的结构模型%Determining Structural Models of Biomolecular Complexes Integrating Nuclear Magnetic Resonance, Small-Angle X-ray Scattering and Computational Simulations

    Institute of Scientific and Technical Information of China (English)

    彭俊辉; 赵德彪; 文彬; 张志勇

    2015-01-01

    Structural biology has been paying more attention on biomolecular complexes over the past decades, since they are crucial for many biological processes. Among these techniques for structural determination, nuclear magnetic resonance (NMR) has its advantage when dealing with biomolecules with high flexibility in solution. Small-angle X-ray scattering (SAXS) is a very important complementary technique that provides information on global shape of biomolecules. For biomolecular complexes, it can be much easier to determine atomic structures of individual subunits through NMR. In addition, NMR can also provide other structural information, such as the interface and orientations between subunits, and long range distance and angular restraints. Therefore, to construct structural models of biomolecular complexes, it would be very appropriate to combine experimental restraints obtained through NMR and low-resolution shape information from SAXS by utilizing computational tools, which is the main topic of this review.%近年来,结构生物学研究越来越注重生物大分子复合物的解析,因为许多重要生物学过程都离不开复合物的参与.溶液核磁共振是目前重要的结构解析方法之一.X射线小角散射(SAXS)作为一种新的结构生物学实验手段,近年来发展迅速.SAXS 能提供生物大分子复合物的较低分辨率结构信息,而核磁共振能解析复合物中各个亚基的原子分辨率结构.此外,通过核磁共振还能得到亚基之间的界面、取向以及距离信息.因此近年来通过计算机模拟,整合核磁共振和 SAXS 不同分辨率的结构信息,可以用来搭建生物大分子复合物的结构模型.该综述重点介绍这方面的研究进展.

  15. Modeling the effect of small-scale magnetic turbulence on the X-ray properties of Pulsar Wind Nebulae

    Science.gov (United States)

    Bucciantini, N.; Bandiera, R.; Olmi, B.; Del Zanna, L.

    2017-10-01

    Pulsar Wind Nebulae (PWNe) constitute an ideal astrophysical environment to test our current understanding of relativistic plasma processes. It is well known that magnetic fields play a crucial role in their dynamics and emission properties. At present, one of the main issues concerns the level of magnetic turbulence present in these systems, which in the absence of space resolved X-ray polarization measures cannot be directly constrained. In this work, we investigate, for the first time using simulated synchrotron maps, the effect of a small-scale fluctuating component of the magnetic field on the emission properties in X-ray. We illustrate how to include the effects of a turbulent component in standard emission models for PWNe and which consequences are expected in terms of net emissivity and depolarization, showing that the X-ray surface brightness maps can provide already some rough constraints. We then apply our analysis to the Crab and Vela nebulae and by comparing our model with Chandra and Vela data, we found that the typical energies in the turbulent component of the magnetic field are about 1.5-3 times the one in the ordered field.

  16. Soft x-ray microscopy - a powerful analytical tool to image magnetism down to fundamental length and times scales

    Energy Technology Data Exchange (ETDEWEB)

    Fischer, Peter

    2008-08-01

    The magnetic properties of low dimensional solid state matter is of the utmost interest both scientifically as well as technologically. In addition to the charge of the electron which is the base for current electronics, by taking into account the spin degree of freedom in future spintronics applications open a new avenue. Progress towards a better physical understanding of the mechanism and principles involved as well as potential applications of nanomagnetic devices can only be achieved with advanced analytical tools. Soft X-ray microscopy providing a spatial resolution towards 10nm, a time resolution currently in the sub-ns regime and inherent elemental sensitivity is a very promising technique for that. This article reviews the recent achievements of magnetic soft X-ray microscopy by selected examples of spin torque phenomena, stochastical behavior on the nanoscale and spin dynamics in magnetic nanopatterns. The future potential with regard to addressing fundamental magnetic length and time scales, e.g. imaging fsec spin dynamics at upcoming X-ray sources is pointed out.

  17. Dissecting X-Ray Raman Resonances Using Four-Wave Mixing

    Energy Technology Data Exchange (ETDEWEB)

    Biggs, Jason D.; Zhang, Yu; Healion, Daniel; Govind, Niranjan; Shaul, Mukamel; Chergui, M.; Taylor, A.; Cundiff, S.; de Vivie-Riedle, R.; Yamagouchi, K.

    2013-01-01

    The stimulated x-ray Raman signal has been calculated for the amino acid cysteine using broadband (FWHM ≃14.2eV, 128 as) pulses tuned to the nitrogen K-edge. Peaks correspond to those valence excited states and reveal electronic Frank-Condon overlaps between canonical valence orbitals and relaxed orbitals in the presence of the core hole. The coupling between excited states with valence- and core-holes is further explored using a coherent, wave-vector matched photon echo technique, where it is possible to eliminate stimulated emission and excited-state absorption by taking the waiting time to be longer the lifetime of the core hole (~ 7:1 fs for nitrogen).

  18. Dissecting X-Ray Raman Resonances Using Four-Wave Mixing

    Directory of Open Access Journals (Sweden)

    Govind Niranjan

    2013-03-01

    Full Text Available The stimulated x-ray Raman signal has been calculated for the amino acid cysteine using broadband (FWHM ≃14.2eV, 128 as pulses tuned to the nitrogen K-edge. Peaks correspond to those valence excited states and reveal electronic Frank-Condon overlaps between canonical valence orbitals and relaxed orbitals in the presence of the core hole. The coupling between excited states with valence- and core-holes is further explored using a coherent, wave-vector matched photon echo technique, where it is possible to eliminate stimulated emission and excited-state absorption by taking the waiting time to be longer the lifetime of the core hole (∼ 7:1 fs for nitrogen.

  19. Resonant X-ray diffraction using high-resolution image-plate data

    Energy Technology Data Exchange (ETDEWEB)

    Ehrenberg, H.; Knapp, M.; Hartmann, T.; Fuess, H. [Technische Hochschule Darmstadt (Germany). Fachbereich Materialwissenschaften; Wroblewski, T. [Hamburger Synchrotron Lab., Hamburg (Germany)

    2000-06-01

    The experimental setup for the collection of synchrotron X-ray powder diffraction data from samples with high absorption ({mu}R > 10) is described. It consists of a combination of a vacuum chamber with an image-plate system. A numerical absorption correction for the applied geometry has been derived and the data were corrected accordingly. Values for f'(Er) and f{sup ''}(Er) were refined from eight measurements on Er{sub 5}Re{sub 2}O{sub 12} above and below the Er L{sub III} absorption edge. Successful refinement of the crystallographic data has verified the high quality of the collected intensities. (orig.)

  20. Magnetism of unconventional nanoscaled materials. An X-ray circular dichroism and muon spin rotation study

    Energy Technology Data Exchange (ETDEWEB)

    Tietze, Thomas Hermann

    2014-12-15

    The physical properties of nanoparticles deviate strongly from its bulk counterparts. In particular, the magnetic properties change strongly due to an elevated number of surface compared to bulk atoms. As a consequence the orbital magnetic moment in nanoparticles as well as the magnetic anisotropy is enhanced. Therefore, such nanoparticles have great potential in e.g. next generation high density data storage devices. A promising way to realize such devices is to deposit nanoparticles on graphene. Depending on the preparation conditions the templated growth of nanocluster arrays with different particle size and shape is possible. Since graphene possesses outstanding properties as well it is congruous to combine the advantages of both systems and to investigate its principle properties in more detail. Thus, one part of this work is dedicated to the size and shape dependence of electronic and magnetic properties of Ni nanoclusters on graphene. The magnetic properties were investigated using X-ray Magnetic Circular Dichroism (XMCD). From the corresponding absorption spectra, the electronic structure and the nanoparticle substrate interaction could be determined. Two sets of nanoparticles were investigated, with triangular and spherical shape. For each set the size was varied. Nonmagnetic absorption spectra indicate a strong interaction between the Ni nanoclusters and the graphene substrate. The integrated absorption signal which is a measure of the number of unoccupied states in the Ni d shell decreases strongly with decreasing cluster size. This means an enhanced occupancy of the Ni d states, most likely caused by charge transfer at the Ni nanocluster/graphene interface. As a consequence the magnetic moment was much smaller than expected for nanoclusters for all samples investigated. The smallest value obtained was only 50% of the respective bulk magnetic moment. The magnetic moment increases disproportionally and converges towards bulk properties above 2 ML. No

  1. Multi-band study of a new asynchronous magnetic cataclysmic variable and a flaring X-ray source

    CERN Document Server

    Rea, N; Esposito, P; D'Avanzo, P; de Martino, D; Israel, G L; Torres, D F; Campana, S; Belloni, T M; Papitto, A; Masetti, N; Carrasco, L; Possenti, A; Wieringa, M; Wilhelmi, E De Ona; Li, J; Bozzo, E; Ferrigno, C; Linares, M; Tauris, T M; Hernanz, M; Ribas, I; Monelli, M; Borghese, A; Baglio, M C; Casares, J

    2016-01-01

    In search for the counterpart to the Fermi-LAT source 3FGL J0838.8-2829, we report on 1) a new magnetic Cataclysmic Variable (mCV), RX J0838-2827, that we identify as an asynchronous system (therefore not associated with this Fermi-LAT source) and 2) on a new X-ray flaring source, XMM J083850.4-282759, that might be tentatively identified as new candidate Transitional Millisecond Pulsar, possibly associated with the gamma-ray source. We observed the field in the X-ray band with Swift, twice with XMM-Newton, as well as performed infrared, optical (with OAGH, ESO-NTT and IAC80) and radio (ATCA) observations, and we report on archival INTEGRAL observations. RX J0838-2827 is extremely variable in the X-ray and optical bands, and timing analysis reveals the presence of several periodicities modulating its X-ray and optical emission. The most evident modulations are interpreted as due to the binary system orbital period of ~1.64hr and the white dwarf spin period of ~1.47hr. Furthermore, a strong flux modulation at ...

  2. X-ray-scattering study of copper magnetism in nonsuperconducting PrBa2Cu3O6.92

    DEFF Research Database (Denmark)

    Hill, J.P.; McMorrow, D.F.; Boothroyd, A.T.

    2000-01-01

    X-ray magnetic scattering from ordered Cu spins has been observed in a high-T-c compound. The measurements were made on the anomalous cuprate PrBa2Cu3O6.92 with x-ray photon energies tuned in the vicinity of the Cu K edge. The high wave-vector resolution enabled us to observe an incommensurate...... double-Q Cu spin structure below T-Pr = 19 K that forms as a result of coupling between the magnetically ordered Cu and Pr sublattices. Above T-Pr, the Cu ordering is commensurate, ruling out static spin-charge stripe order as an explanation for the absence of superconductivity in this material....

  3. Spin state transition in LaCoO3 studied using soft x-ray absorption spectroscopy and magnetic circular dichroism.

    Science.gov (United States)

    Haverkort, M W; Hu, Z; Cezar, J C; Burnus, T; Hartmann, H; Reuther, M; Zobel, C; Lorenz, T; Tanaka, A; Brookes, N B; Hsieh, H H; Lin, H-J; Chen, C T; Tjeng, L H

    2006-10-27

    Using soft x-ray absorption spectroscopy and magnetic circular dichroism at the Co-L(2,3) edge, we reveal that the spin state transition in LaCoO3 can be well described by a low-spin ground state and a triply degenerate high-spin first excited state. From the temperature dependence of the spectral line shapes, we find that LaCoO3 at finite temperatures is an inhomogeneous mixed-spin state system. It is crucial that the magnetic circular dichroism signal in the paramagnetic state carries a large orbital momentum. This directly shows that the currently accepted low- or intermediate-spin picture is at variance. Parameters derived from these spectroscopies fully explain existing magnetic susceptibility, electron spin resonance, and inelastic neutron data.

  4. In vivo tumour extracellular pH monitoring using electron paramagnetic resonance: the effect of X-ray irradiation.

    Science.gov (United States)

    Goodwin, Jonathan; Yachi, Katsuya; Nagane, Masaki; Yasui, Hironobu; Miyake, Yusuke; Inanami, Osamu; Bobko, Andrey A; Khramtsov, Valery V; Hirata, Hiroshi

    2014-04-01

    The in vivo quantification of extracellular pH (pHe ) in tumours may provide a useful biomarker for tumour cell metabolism. In this study, we assessed the viability of continuous-wave electron paramagnetic resonance (CW-EPR) spectroscopy with a pH-sensitive nitroxide for the measurement of extracellular tumour pH in a mouse model. CW-EPR spectroscopy (750 MHz) of C3H HeJ mice hind leg squamous cell tumour was performed after intravenous tail vein injection of pH-sensitive nitroxide (R-SG, 2-(4-((2-(4-amino-4-carboxybutanamido)-3-(carboxymethylamino)-3-oxoproylthio)methyl)phenyl)-4-pyrrolidino-2,5,5-triethyl-2,5-dihydro-1Н-imidazol-1-oxyl) during stages of normal tumour growth and in response to a single 10-Gy dose of X-ray irradiation. An inverse relationship was observed between tumour volume and pHe value, whereby, during normal tumour growth, a constant reduction in pHe was observed. This relationship was disrupted by X-ray irradiation and, from 2-3 days post-exposure, a transitory increase in pHe was observed. In this study, we demonstrated the viability of CW-EPR spectroscopy using R-SG nitroxide to obtain high-sensitivity pH measurements in a mouse tumour model with an accuracy of <0.1 pH units. In addition, the measured changes in pHe in response to X-ray irradiation suggest that this may offer a useful method for the assessment of the physiological change in response to existing and novel cancer therapies. Copyright © 2014 John Wiley & Sons, Ltd.

  5. SMALL VOLUME LONG PULSE X RAY PREIONISED XeCl LASER WITH DOUBLE DISCHARGE AND FAST FERRITE MAGNETIC SWITCH

    OpenAIRE

    J. Hueber; Kobhio, M.; Fontaine, B.; Delaporte, Ph.; Sentis, M.; Forestier, B.

    1991-01-01

    Experimental results obtained with a high efficiency small volume long pulse X-Ray preionised XeCl laser with double discharge and very fast ferrite magnetic switch are presented and compared with the results given by a new XeCl laser numerical self consistant model. The model takes into account most recent kinetic data and time variation of discharge impedence and switch inductance. There is a good agreement between experiment and model on electrical and laser parameters for typical conditions.

  6. High-Resolution X-ray Emission and X-ray Absorption Spectroscopy

    OpenAIRE

    de Groot, F. M. F.

    2001-01-01

    In this review, high-resolution X-ray emission and X-ray absorption spectroscopy will be discussed. The focus is on the 3d transition-metal systems. To understand high-resolution X-ray emission and reso-nant X-ray emission, it is first necessary to spend some time discussing the X-ray absorption process. Section II discusses 1s X-ray absorption, i.e., the K edges, and section III deals with 2p X-ray absorption, the L edges. X-ray emission is discussed in, respectively, the L edges. X-ray emis...

  7. Revisiting the Magnetic and Spin Evolution of Two Young X-ray Pulsars

    Science.gov (United States)

    Ferdman, Robert; Kaspi, Victoria M.; Archibald, Robert Frederic

    2014-08-01

    We present results from timing analysis of two young X-ray pulsars found in the large Magellanic Cloud: the Crab-like energetic pulsar PSR B0540-69 and the so-called "big glitcher", PSR J0537-6910. In both cases, we analyze data taken with the Rossi X-ray Timing Explorer. This work extends the published data sets for these pulsars by approximately doubling their respective data spans. We revisit the glitching activity of these neutron stars, particularly that of PSR J0537-6910, determine more precise glitch and spin parameters, and discuss the implications for the spin and magnetospheric evolution of these interesting pulsars.

  8. Spin period change and the magnetic fields of neutron stars in Be X-ray binaries in the SMC

    Directory of Open Access Journals (Sweden)

    Klus H.

    2014-01-01

    Full Text Available We report on the long term average spin period, rate of change of spin period and X-ray luminosity during outbursts for 42 Be X-ray binary systems in the Small Magellanic Cloud. We also collect and calculate parameters of each system and use this data to determine that all systems contain a neutron star which is accreting via a disc, rather than a wind, and that if these neutron stars are near spin equilibrium, then over half of them, including all with spin periods over about 100 seconds, have magnetic fields over the quantum critical level of 4.4×1013 G. If these neutron stars are not close to spin equilibrium, then their magnetic fields are inferred to be much lower, on the order of 106-1010 G, comparable to the fields of neutron stars in low mass X-ray binaries. Both results are unexpected and have implications for the rate of magnetic field decay and the isolated neutron star population.

  9. New structural studies of liquid crystal by reflectivity and resonant X-ray diffraction; Nouvelles etudes structurales de cristaux liquides par reflectivite et diffraction resonante des rayons X

    Energy Technology Data Exchange (ETDEWEB)

    Fernandes, P

    2007-04-15

    This memory presents three structural studies of smectic Liquid Crystals by reflectivity and resonant diffraction of X-rays. It is divided in five chapters. In the first a short introduction to Liquid Crystals is given. In particular, the smectic phases that are the object of this study are presented. The second chapter is consecrated to the X-ray experimental techniques that were used in this work. The three last chapters present the works on which this thesis can be divided. Chapter three demonstrates on free-standing films of MHPOBC (historic liquid crystal that possesses the antiferroelectric sub-phases) the possibility to extend the technique of resonant X-ray diffraction to liquid crystals without resonant element. In the fourth chapter the structure of the B{sub 2} liquid crystal phase of bent-core molecules (or banana molecules) is elucidated by using resonant X-ray diffraction combined with polarization analysis of the diffracted beam. A model of the polarization of the resonant beam diffracted by four different structures proposed for the B{sub 2} phase is developed in this chapter. In the fifth chapter a smectic binary mixture presenting a very original critical point of phase separation is studied by X-ray reflectivity and optical microscopy. A concentration gradient in the direction perpendicular to the plane of the film seems to be induced by the free-standing film geometry. The results of a simplified model of the system are compatible with this interpretation.

  10. X-ray magnetic circular dichroism study of Dy-doped Bi2Te3 topological insulator thin films

    Science.gov (United States)

    Figueroa, A. I.; Baker, A. A.; Harrison, S. E.; Kummer, K.; van der Laan, G.; Hesjedal, T.

    2017-01-01

    Magnetic doping of topological insulators (TIs) is crucial for unlocking novel quantum phenomena, paving the way for spintronics applications. Recently, we have shown that doping with rare earth ions introduces large magnetic moments and allows for high doping concentrations without the loss of crystal quality, however no long range magnetic order was observed. In Dy-doped Bi2Te3 we found a band gap opening above a critical doping concentration, despite the paramagnetic bulk behavior. Here, we present a surface-sensitive x-ray magnetic circular dichroism (XMCD) study of an in situ cleaved film in the cleanest possible environment. The Dy M4,5 absorption spectra measured with circularly polarized x-rays are fitted using multiplet calculations to obtain the effective magnetic moment. Arrott-Noakes plots, measured by the Dy M5 XMCD as a function of field at low temperatures, give a negative transition temperature. The evaporation of a ferromagnetic Co thin film did not introduce ferromagnetic ordering of the Dy dopants either; instead a lowering of the transition temperature was observed, pointing towards an antiferromagnetic ordering scenario. This result shows that there is a competition between the magnetic exchange interaction and the Zeeman interaction. The latter favors the Co and Dy magnetic moments to be both aligned along the direction of the applied magnetic field, while the exchange interaction is minimized if the Dy and Co atoms are antiferromagnetically coupled, as in zero applied field.

  11. Quadrupole moments in chiral material DyFe3(BO3)4 observed by resonant x-ray diffraction

    Science.gov (United States)

    Nakajima, Hiroshi; Usui, Tomoyasu; Joly, Yves; Suzuki, Motohiro; Wakabayashi, Yusuke; Kimura, Tsuyoshi; Tanaka, Yoshikazu

    2016-04-01

    By means of circularly polarized x rays at the Dy L3 and Fe K absorption edges, the chiral structure of the electric quadrupole was investigated for a single crystal of DyFe3(BO3)4, in which both Dy and Fe ions exhibit a spiral arrangement. The integrated intensity of the resonant x-ray diffraction of space-group forbidden reflections 004 and 005 is interpreted within the electric dipole transitions from Dy 2 p3/2 to 5 d and Fe 1 s to 4 p , respectively. We have confirmed that the handedness of the crystal observed at Dy L3 and Fe K edges is consistent with that observed at Dy M5 edge reported in a previous study. The electric quadrupole moments of Dy 5 d and Fe 4 p are derived by analyzing the azimuth scans of the diffracted intensity. The temperature profiles of the integrated intensity of 004 at the Dy L3 and the Fe K edges are similar to those of Dy-O and Fe-O bond lengths, while the temperature dependence at the Dy M5 edge does not match the bond-length behavior. The results indicate that the helix chiral orientations of quadrupole moments due to Dy 5 d and Fe 4 p electrons are more strongly coupled to the ligands states than Dy 4 f electrons.

  12. Microscopic Magnetic Properties of the Itinerant Metamagnet UCoAl by X-ray Magnetic Circular Dichroism

    Science.gov (United States)

    Combier, Tristan; Palacio-Morales, Alexandra; Sanchez, Jean-Pierre; Wilhelm, Fabrice; Pourret, Alexandre; Brison, Jean-Pascal; Aoki, Dai; Rogalev, Andrei

    2017-02-01

    The itinerant metamagnet UCoAl has been investigated by high field X-ray magnetic circular dichroism (XMCD) at the U M4,5 and Co K edges. The orbital and spin moments of U at 2.1 K for H || c applied below and above the first order metamagnetic transition field (HM) have been determined. The magnetism of UCoAl is dominated by the U moment. There is no evidence for any change of the orbital to spin moment ratio (˜-2.05) across HM and within the ferromagnetic phase up to 17 T. The possibility of a Fermi surface reconstruction at HM remains an open option. XMCD at the Co K-edge reveals the presence of a small Co 4p-orbital moment parallel to the macroscopic magnetization. In addition, the Co 3d-moment is estimated to be at most 0.1 μB at 17 T. The similar field dependence of the U and Co magnetizations indicates that the Co moment is induced by the U moment.

  13. High orbital angular momentum quantum numbers in the electronic ground states of Fe$_2^+$ and Co$_2^+$ as determined by x-ray absorption and x-ray magnetic circular dichroism spectroscopy

    CERN Document Server

    Zamudio-Bayer, V; Langenberg, A; Lawicki, A; Terasaki, A; Issendorff, B v; Lau, J T

    2015-01-01

    The $^6\\Delta$ electronic ground state of the Co$_2^+$ diatomic molecular cation has been assigned experimentally by x-ray absorption and x-ray magnetic circular dichroism spectroscopy in a cryogenic ion trap. Three candidates, $^6\\Phi$, $^6\\Gamma$, and $^8\\Gamma$, for the electronic ground state of Fe$_2^+$ have been identified. These states carry sizable ground-state orbital angular momenta that disagree with theoretical predictions from multireference configuration interaction and density functional theory. Our results show that the ground states of neutral and cationic diatomic molecules of $3d$ elements cannot be assumed to be connected by a one-electron process.

  14. Origin of (105) Reflection of X-Ray Diffraction and Quantitative Evaluation of Alignment Degree for Sintered Nd-Fe-B Magnets

    Institute of Scientific and Technical Information of China (English)

    HE Ye-Qing; ZHOU Shou-Zeng; ZHANG Zhen-Rong; HAN Bao-Shan

    2001-01-01

    A new method for quantitatively evaluating the alignment degree ofsintered Nd-FeB magnets by x-ray diffraction spectra has been proposed. It has been experimentally revealed that the strong (105) reflection existing in almost all x-ray diffraction spectra of sintered Nd-FeB magnets stems from the misalignment grains whose easy axes are at an angle of 15.5° with respect to the orientated direction of the magnet.

  15. MAGNETIC-X-RAY DICHROISM - GENERAL FEATURES OF DIPOLAR AND QUADRUPOLAR SPECTRA

    NARCIS (Netherlands)

    CARRA, P; KONIG, H; THOLE, BT; ALTARELLI, M

    1993-01-01

    Sum rules are derived for dipolar linear and quadrupolar circular dichroism in the X-ray region. They relate the intensity of the dichroic signal to the ground state expectation values of orbital and spin dependent effective operators, which act on the valence electrons. The results obtained are

  16. Crystalline, mixed-valence manganese analogue of prussian blue: magnetic, spectroscopic, X-ray and neutron diffraction studies.

    Science.gov (United States)

    Franz, Patrick; Ambrus, Christina; Hauser, Andreas; Chernyshov, Dmitry; Hostettler, Marc; Hauser, Jürg; Keller, Lukas; Krämer, Karl; Stoeckli-Evans, Helen; Pattison, Philip; Bürgi, Hans-Beat; Decurtins, Silvio

    2004-12-22

    The compound of stoichiometry Mn(II)3[Mn(III)(CN)6]2.zH2O (z = 12-16) (1) forms air-stable, transparent red crystals. Low-temperature single crystal optical spectroscopy and single crystal X-ray diffraction provide compelling evidence for N-bonded high-spin manganese(II), and C-bonded low-spin manganese(III) ions arranged in a disordered, face-centered cubic lattice analogous to that of Prussian Blue. X-ray and neutron diffraction show structured diffuse scattering indicative of partially correlated (rather than random) substitutions of [Mn(III)(CN)6] ions by (H2O)6 clusters. Magnetic susceptibility measurements and elastic neutron scattering experiments indicate a ferrimagnetic structure below the critical temperature Tc = 35.5 K.

  17. X-Ray Magnetic Dichroism of Antiferromagnet Fe2O3 : The Orientation of Magnetic Moments Observed by Fe 2p X-Ray Absorption Spectroscopy

    NARCIS (Netherlands)

    Kuiper, Pieter; Searle, Barry G.; Rudolf, Petra; Tjeng, L.H.; Chen, C.T.

    1993-01-01

    We report strong magnetic linear dichroism at the Fe L2,3 edge of the antiferromagnet Fe2O3 (hematite). The relative difference in absorption for light polarized parallel and perpendicular to the magnetic moment is as high as 40% at the Fe L2 edge. The spectra are in excellent agreement with

  18. Melting of Bi sublattice in nanosized BiFeO3 Perovskite by resonant X-ray diffraction.

    Science.gov (United States)

    Petkov, V; Selbach, S M; Einarsrud, M-A; Grande, T; Shastri, S D

    2010-10-29

    Free-standing BiFeO3 perovskite particles with a size ranging from polycrystalline bulk down to 5 nm have been studied by high-energy resonant (Bi K edge) x-ray diffraction coupled to differential atomic pair distribution function analysis. Nanosized BiFeO3 particles are found to exhibit extra, i.e., beyond the usual thermal, structural disorder that increases progressively with diminishing their size. In particles of size smaller than approximately 18 nm the disorder destroys the structural coherence of the Bi sublattice and disturbs that of the Fe-based sublattice in the perovskite structure, substantially affecting the magnetoelectric properties it carries. The new structural information helps better understand the unusual behavior of perovskites structured at the nanoscale.

  19. Quantifying point defects in Cu2ZnSn(S,Se)4 thin films using resonant x-ray diffraction

    Energy Technology Data Exchange (ETDEWEB)

    Stone, Kevin H. [Stanford Synchrotron Radiation Lightsource, SLAC National Accelerator Laboratory, Menlo Park, California 94025, USA; Christensen, Steven T. [National Renewable Energy Laboratory, Golden, Colorado 80401, USA; Harvey, Steven P. [National Renewable Energy Laboratory, Golden, Colorado 80401, USA; Teeter, Glenn [National Renewable Energy Laboratory, Golden, Colorado 80401, USA; Repins, Ingrid L. [National Renewable Energy Laboratory, Golden, Colorado 80401, USA; Toney, Michael F. [Stanford Synchrotron Radiation Lightsource, SLAC National Accelerator Laboratory, Menlo Park, California 94025, USA

    2016-10-17

    Cu 2ZnSn(S,Se)4 is an interesting, earth abundant photovoltaic material, but has suffered from low open circuit voltage. To better understand the film structure, we have measured resonant x-ray diffraction across the Cu and Zn K-edges for the device quality thin films of Cu 2ZnSnS4 (8.6% efficiency) and Cu 2ZnSn(S,Se)4 (3.5% efficiency). This approach allows for the confirmation of the underlying kesterite structure and quantification of the concentration of point defects and vacancies on the Cu, Zn, and Sn sublattices. Rietveld refinement of powder diffraction data collected at multiple energies is used to determine that there exists a high level of Cu Zn and Zn Cu defects on the 2c and 2d Wyckoff positions. We observe a significantly lower concentration of Zn Sn defects and Cu or Zn vacancies.

  20. Quantifying covalent interactions with resonant inelastic soft X-ray scattering: Case study of Ni2+ aqua complex

    Science.gov (United States)

    Kunnus, K.; Josefsson, I.; Schreck, S.; Quevedo, W.; Miedema, P. S.; Techert, S.; de Groot, F. M. F.; Föhlisch, A.; Odelius, M.; Wernet, Ph.

    2017-02-01

    We analyze the effects of covalent interactions in Ni 2p3d resonant inelastic X-ray scattering (RIXS) spectra from aqueous Ni2+ ions and find that the relative RIXS intensities of ligand-to-metal charge-transfer final states with respect to the ligand-field final states reflect the covalent mixing between Ni 3d and water orbitals. Specifically, the experimental intensity ratio at the Ni L3-edge allows to determine that the Ni 3d orbitals have on average 5.5% of water character. We propose that 2p3d RIXS at the Ni L3-edge can be utilized to quantify covalency in Ni complexes without the use of external references or simulations.

  1. Quantifying point defects in Cu2ZnSn(S,Se)4 thin films using resonant x-ray diffraction

    Science.gov (United States)

    Stone, Kevin H.; Christensen, Steven T.; Harvey, Steven P.; Teeter, Glenn; Repins, Ingrid L.; Toney, Michael F.

    2016-10-01

    Cu2ZnSn(S,Se)4 is an interesting, earth abundant photovoltaic material, but has suffered from low open circuit voltage. To better understand the film structure, we have measured resonant x-ray diffraction across the Cu and Zn K-edges for the device quality thin films of Cu2ZnSnS4 (8.6% efficiency) and Cu2ZnSn(S,Se)4 (3.5% efficiency). This approach allows for the confirmation of the underlying kesterite structure and quantification of the concentration of point defects and vacancies on the Cu, Zn, and Sn sublattices. Rietveld refinement of powder diffraction data collected at multiple energies is used to determine that there exists a high level of CuZn and ZnCu defects on the 2c and 2d Wyckoff positions. We observe a significantly lower concentration of ZnSn defects and Cu or Zn vacancies.

  2. Deep X-Ray Lithography Based Fabrication of Rare-Earth Based Permanent Magnets and their Applications to Microactuators

    Energy Technology Data Exchange (ETDEWEB)

    Christenson, T.R.; Garino, T.J.; Venturini, E.L.

    1999-01-27

    Precision high aspect-ratio micro molds constructed by deep x-ray lithography have been used to batch fabricate accurately shaped bonded rare-earth based permanent magnets with features as small as 5 microns and thicknesses up to 500 microns. Maximum energy products of up to 8 MGOe have been achieved with a 20%/vol. epoxy bonded melt-spun isotropic Nd2Fe14b powder composite. Using individually processed sub- millimeter permanent sections multipole rotors have been assembled. Despite the fact that these permanent magnet structures are small, their magnetic field producing capability remains the same as at any scale. Combining permanent magnet structures with soft magnetic materials and micro-coils makes possible new and more efficient magnetic microdevices.

  3. Nature of magnetic coupling between Mn ions in as-grown Ga$_{1-x}$Mn$_{x}$As studied by x-ray magnetic circular dichroism

    OpenAIRE

    Takeda, Y.; Kobayashi, M.; Okane, T.; Ohkochi, T.; Okamoto, J.; Saitoh, Y; Kobayashi, K.; Yamagami, H.; Fujimori, A.; Tanaka, A.; Okabayashi, J.; Oshima, M.; Ohya, S; Hai, P.N.; Tanaka, M.

    2008-01-01

    The magnetic properties of as-grown Ga$_{1-x}$Mn$_{x}$As have been investigated by the systematic measurements of temperature and magnetic field dependent soft x-ray magnetic circular dichroism (XMCD). The {\\it intrinsic} XMCD intensity at high temperatures obeys the Curie-Weiss law, but residual spin magnetic moment appears already around 100 K, significantly above Curie temperature ($T_C$), suggesting that short-range ferromagnetic correlations are developed above $T_C$. The present results...

  4. Identification of an organic semiconductor superlattice structure of pentacene and perfluoro-pentacene through resonant and non-resonant X-ray scattering

    Energy Technology Data Exchange (ETDEWEB)

    Kowarik, S.; Weber, C. [Humboldt-Universität zu Berlin, Institut für Physik, Newtonstr. 15, 12489 Berlin (Germany); Hinderhofer, A.; Gerlach, A.; Schreiber, F. [Universität Tübingen, Institut für Angewandte Physik, Auf der Morgenstelle 10, 72076 Tübingen (Germany); Wang, C.; Hexemer, A. [Advanced Light Source, Lawrence Berkeley National Laboratory, Berkeley, CA 94720 (United States); Leone, S. R. [Departments of Chemistry and Physics, University of California, and Lawrence Berkeley National Laboratory, Berkeley, CA 94720 (United States)

    2015-11-15

    Highly crystalline and stable molecular superlattices are grown with the smallest possible stacking period using monolayers (MLs) of the organic semiconductors pentacene (PEN) and perfluoro-pentacene (PFP). Superlattice reflections in X-ray reflectivity and their energy dependence in resonant soft X-ray reflectivity measurements show that PFP and PEN MLs indeed alternate even though the coherent ordering is lost after ∼ 4 ML. The observed lattice spacing of 15.9 Å in the superlattice is larger than in pure PEN and PFP films, presumably because of more upright standing molecules and lack of interdigitation between the incommensurate crystalline PEN and PFP layers. The findings are important for the development of novel organic quantum optoelectronic devices.

  5. Identification of an organic semiconductor superlattice structure of pentacene and perfluoro-pentacene through resonant and non-resonant X-ray scattering

    Directory of Open Access Journals (Sweden)

    S. Kowarik

    2015-11-01

    Full Text Available Highly crystalline and stable molecular superlattices are grown with the smallest possible stacking period using monolayers (MLs of the organic semiconductors pentacene (PEN and perfluoro-pentacene (PFP. Superlattice reflections in X-ray reflectivity and their energy dependence in resonant soft X-ray reflectivity measurements show that PFP and PEN MLs indeed alternate even though the coherent ordering is lost after ∼ 4 ML. The observed lattice spacing of 15.9 Å in the superlattice is larger than in pure PEN and PFP films, presumably because of more upright standing molecules and lack of interdigitation between the incommensurate crystalline PEN and PFP layers. The findings are important for the development of novel organic quantum optoelectronic devices.

  6. Numerical Solution of the Radiative Transfer Equation: X-Ray Spectral Formation from Cylindrical Accretion onto a Magnetized Neutron Star

    Science.gov (United States)

    Fairnelli, R.; Ceccobello, C.; Romano, P.; Titarchuk, L.

    2011-01-01

    Predicting the emerging X-ray spectra in several astrophysical objects is of great importance, in particular when the observational data are compared with theoretical models. This requires developing numerical routines for the solution of the radiative transfer equation according to the expected physical conditions of the systems under study. Aims. We have developed an algorithm solving the radiative transfer equation in the Fokker-Planck approximation when both thermal and bulk Comptonization take place. The algorithm is essentially a relaxation method, where stable solutions are obtained when the system has reached its steady-state equilibrium. Methods. We obtained the solution of the radiative transfer equation in the two-dimensional domain defined by the photon energy E and optical depth of the system pi using finite-differences for the partial derivatives, and imposing specific boundary conditions for the solutions. We treated the case of cylindrical accretion onto a magnetized neutron star. Results. We considered a blackbody seed spectrum of photons with exponential distribution across the accretion column and for an accretion where the velocity reaches its maximum at the stellar surface and at the top of the accretion column, respectively. In both cases higher values of the electron temperature and of the optical depth pi produce flatter and harder spectra. Other parameters contributing to the spectral formation are the steepness of the vertical velocity profile, the albedo at the star surface, and the radius of the accretion column. The latter parameter modifies the emerging spectra in a specular way for the two assumed accretion profiles. Conclusions. The algorithm has been implemented in the XPEC package for X-ray fitting and is specifically dedicated to the physical framework of accretion at the polar cap of a neutron star with a high magnetic field (approx > 10(exp 12) G). This latter case is expected to be of typical accreting systems such as X-ray

  7. Kissing G domains of MnmE monitored by X-ray crystallography and pulse electron paramagnetic resonance spectroscopy.

    Science.gov (United States)

    Meyer, Simon; Böhme, Sabine; Krüger, André; Steinhoff, Heinz-Jürgen; Klare, Johann P; Wittinghofer, Alfred

    2009-10-01

    MnmE, which is involved in the modification of the wobble position of certain tRNAs, belongs to the expanding class of G proteins activated by nucleotide-dependent dimerization (GADs). Previous models suggested the protein to be a multidomain protein whose G domains contact each other in a nucleotide dependent manner. Here we employ a combined approach of X-ray crystallography and pulse electron paramagnetic resonance (EPR) spectroscopy to show that large domain movements are coupled to the G protein cycle of MnmE. The X-ray structures show MnmE to be a constitutive homodimer where the highly mobile G domains face each other in various orientations but are not in close contact as suggested by the GDP-AlF(x) structure of the isolated domains. Distance measurements by pulse double electron-electron resonance (DEER) spectroscopy show that the G domains adopt an open conformation in the nucleotide free/GDP-bound and an open/closed two-state equilibrium in the GTP-bound state, with maximal distance variations of 18 A. With GDP and AlF(x), which mimic the transition state of the phosphoryl transfer reaction, only the closed conformation is observed. Dimerization of the active sites with GDP-AlF(x) requires the presence of specific monovalent cations, thus reflecting the requirements for the GTPase reaction of MnmE. Our results directly demonstrate the nature of the conformational changes MnmE was previously suggested to undergo during its GTPase cycle. They show the nucleotide-dependent dynamic movements of the G domains around two swivel positions relative to the rest of the protein, and they are of crucial importance for understanding the mechanistic principles of this GAD.

  8. Kissing G domains of MnmE monitored by X-ray crystallography and pulse electron paramagnetic resonance spectroscopy.

    Directory of Open Access Journals (Sweden)

    Simon Meyer

    2009-10-01

    Full Text Available MnmE, which is involved in the modification of the wobble position of certain tRNAs, belongs to the expanding class of G proteins activated by nucleotide-dependent dimerization (GADs. Previous models suggested the protein to be a multidomain protein whose G domains contact each other in a nucleotide dependent manner. Here we employ a combined approach of X-ray crystallography and pulse electron paramagnetic resonance (EPR spectroscopy to show that large domain movements are coupled to the G protein cycle of MnmE. The X-ray structures show MnmE to be a constitutive homodimer where the highly mobile G domains face each other in various orientations but are not in close contact as suggested by the GDP-AlF(x structure of the isolated domains. Distance measurements by pulse double electron-electron resonance (DEER spectroscopy show that the G domains adopt an open conformation in the nucleotide free/GDP-bound and an open/closed two-state equilibrium in the GTP-bound state, with maximal distance variations of 18 A. With GDP and AlF(x, which mimic the transition state of the phosphoryl transfer reaction, only the closed conformation is observed. Dimerization of the active sites with GDP-AlF(x requires the presence of specific monovalent cations, thus reflecting the requirements for the GTPase reaction of MnmE. Our results directly demonstrate the nature of the conformational changes MnmE was previously suggested to undergo during its GTPase cycle. They show the nucleotide-dependent dynamic movements of the G domains around two swivel positions relative to the rest of the protein, and they are of crucial importance for understanding the mechanistic principles of this GAD.

  9. Three-dimensional microstructural investigation of high magnetization nano-micro composite fluids using x-ray microcomputed tomography

    Science.gov (United States)

    Borbáth, T.; Borbáth, I.; Günther, S.; Marinica, O.; Vékás, L.; Odenbach, S.

    2014-05-01

    X-ray microcomputed tomography was used in a three-dimensional investigation of the microstructure of suspensions of multi-domain soft iron particles in magnetic nanofluids. The measurements were performed using two different approaches: with the sample kept frozen, and with the sample under the effect of an external magnetic field. Results show that even a relatively low magnetic field gradient drives the micron-sized iron particles towards the stronger field and thus leads to a redistribution of the ferromagnetic particles in the magnetic nanofluid. Three-dimensional images of the internal microstructure of the composite magnetizable fluid (CMF) were obtained not only for the nano-micro composite system placed in a closed sample holder, but also for the spikes formed at the CMF free surface. It was demonstrated that x-ray microcomputed tomography is an efficient way to investigate the distribution and chain formation of ferromagnetic microparticles in a magnetic nanofluid carrier allowing an analysis even at a single particle level.

  10. MAGNETICALLY DRIVEN WINDS FROM DIFFERENTIALLY ROTATING NEUTRON STARS AND X-RAY AFTERGLOWS OF SHORT GAMMA-RAY BURSTS

    Energy Technology Data Exchange (ETDEWEB)

    Siegel, Daniel M.; Ciolfi, Riccardo; Rezzolla, Luciano [Max Planck Institute for Gravitational Physics (Albert Einstein Institute), Am Mühlenberg 1, D-14476 Potsdam-Golm (Germany)

    2014-04-10

    Besides being among the most promising sources of gravitational waves, merging neutron star binaries also represent a leading scenario to explain the phenomenology of short gamma-ray bursts (SGRBs). Recent observations have revealed a large subclass of SGRBs with roughly constant luminosity in their X-ray afterglows, lasting 10-10{sup 4} s. These features are generally taken as evidence of a long-lived central engine powered by the magnetic spin-down of a uniformly rotating, magnetized object. We propose a different scenario in which the central engine powering the X-ray emission is a differentially rotating hypermassive neutron star (HMNS) that launches a quasi-isotropic and baryon-loaded wind driven by the magnetic field, which is built-up through differential rotation. Our model is supported by long-term, three-dimensional, general-relativistic, and ideal magnetohydrodynamic simulations, showing that this isotropic emission is a very robust feature. For a given HMNS, the presence of a collimated component depends sensitively on the initial magnetic field geometry, while the stationary electromagnetic luminosity depends only on the magnetic energy initially stored in the system. We show that our model is compatible with the observed timescales and luminosities and express the latter in terms of a simple scaling relation.

  11. X-ray absorption spectroscopy and magnetic circular dichroism studies of L1{sub 0}-Mn-Ga thin films

    Energy Technology Data Exchange (ETDEWEB)

    Glas, M., E-mail: mglas@physik.uni-bielefeld.de; Sterwerf, C.; Schmalhorst, J. M.; Reiss, G. [Thin Films and Physics of Nanostructures, Bielefeld University, Bielefeld (Germany); Ebke, D. [Thin Films and Physics of Nanostructures, Bielefeld University, Bielefeld (Germany); Max Planck Institute for Chemical Physics of Solids, Dresden (Germany); Jenkins, C.; Arenholz, E. [ALS Berkeley, California 94720-8229 (United States)

    2013-11-14

    Tetragonally distorted Mn{sub 3−x}Ga{sub x} thin films with 0.1magnetic anisotropy and low magnetization and thus have the potential to serve as electrodes in spin transfer torque magnetic random access memory. Because a direct capping of these films with MgO is problematic due to oxide formation, we examined the influence of a CoFeB interlayer and of two different deposition methods for the MgO barrier on the formation of interfacial Mn-O for Mn{sub 62}Ga{sub 38} by element specific X-ray absorption spectroscopy (XAS) and magnetic circular dichroism (XMCD). A highly textured L1{sub 0} crystal structure of the Mn-Ga films was verified by X-ray diffraction measurements. For samples with e-beam evaporated MgO barrier no evidence for Mn-O was found whereas in samples with magnetron sputtered MgO, Mn-O was detected, even for the thickest interlayer thickness. Both XAS and XMCD measurements showed an increasing interfacial Mn-O amount with decreasing CoFeB interlayer thickness. Additional element specific full hysteresis loops determined an out-of-plane magnetization axis for the Mn and Co, respectively.

  12. X-ray absorption spectroscopy and magnetic circular dichroism studies of L10-Mn-Ga thin films

    Science.gov (United States)

    Glas, M.; Sterwerf, C.; Schmalhorst, J. M.; Ebke, D.; Jenkins, C.; Arenholz, E.; Reiss, G.

    2013-11-01

    Tetragonally distorted Mn3-xGax thin films with 0.1magnetic anisotropy and low magnetization and thus have the potential to serve as electrodes in spin transfer torque magnetic random access memory. Because a direct capping of these films with MgO is problematic due to oxide formation, we examined the influence of a CoFeB interlayer and of two different deposition methods for the MgO barrier on the formation of interfacial Mn-O for Mn62Ga38 by element specific X-ray absorption spectroscopy (XAS) and magnetic circular dichroism (XMCD). A highly textured L10 crystal structure of the Mn-Ga films was verified by X-ray diffraction measurements. For samples with e-beam evaporated MgO barrier no evidence for Mn-O was found whereas in samples with magnetron sputtered MgO, Mn-O was detected, even for the thickest interlayer thickness. Both XAS and XMCD measurements showed an increasing interfacial Mn-O amount with decreasing CoFeB interlayer thickness. Additional element specific full hysteresis loops determined an out-of-plane magnetization axis for the Mn and Co, respectively.

  13. Estudo comparativo dos mecanorreceptores dos discos intervertebrais normais e degenerados da coluna lombar de humanos pela radiografia, ressonância magnética e estudo anatomopatológico Comparative study of normal and degenerated intervertebral discs' mechanoreceptors of human lumar spine X-ray, magnetic resonance and anatomopathologic study

    Directory of Open Access Journals (Sweden)

    Valdeci Manoel de Oliveira

    2007-01-01

    Full Text Available Os autores fizeram um estudo da coluna lombar de humanos, objetivando avaliar e determinar os diferentes tipos de fibras nervosas no disco intervertebral normal e no degenerado. Foram usadas dez colunas lombares de cadáveres com aproximadamente 48 a 72 horas de óbito. As peças foram submetidas a exames de radiografia simples e ressonância magnética. Após os exames, os discos foram classificados em normais e degenerados. Em seguida, foram dissecados, divididos em regiões anterior e posterior, incluídos em parafina e realizado estudo de imuno-histoquímica com a proteína S100. Com o auxílio de um programa de computador Image-Pro Plus (media cybernetics®, as fibras nervosas tiveram seu diâmetro medidos em micrômetros e classificadas em quatro tipos de fibras. Foram encontrados quatro tipos de fibras nervosas nas diferentes regiões discais. O número e o tipo de fibras variaram de acordo com a região e grau de degeneração do disco intervertebral. Concluíram que as fibras do tipo III são mais freqüentes na região anterior; as fibras dos tipos II e IV são mais freqüentes na região posterior, e as fibras do tipo I não apresentaram diferenças entre a região anterior e a posterior; além disso, o disco degenerado tem mais fibras nervosas que o disco normal.The authors conducted a study on human lumbar spine, aiming to assess and determine the different kinds of nervous fibers in normal and degenerated intervertebral discs. Ten cadaver’s lumbar spines with approximately 48 - 72 of death have been used. The pieces were submitted to simple X-ray and magnetic resonance tests. Subsequently to the tests, discs were divided into normal and degenerated. Then, they were dissected, divided into anterior and posterior according to the region, included in paraffin and an immunohistochemical study with S100 protein was performed. With the aid of Image-Pro Plus computer software (media cybernetics ®, nervous fibers’ diameters were

  14. Reaction cell for in situ soft x-ray absorption spectroscopy and resonant inelastic x-ray scattering measurements of heterogeneous catalysis up to 1 atm and 250 °C

    Energy Technology Data Exchange (ETDEWEB)

    Kristiansen, P. T. [Department of Physics and Astronomy, Division of Molecular and Condensed Matter Physics, Uppsala University, Box 516, S-751 20 Uppsala (Sweden); Abteilung Anorganische Chemie, Fritz-Haber-Institut der Max-Planck-Gesellschaft, Faradayweg 4-6, D-14195 Berlin (Germany); Helmholtz-Zentrum Berlin für Materialien und Energie Albert-Einstein-Str. 15, D-12489 Berlin (Germany); Rocha, T. C. R.; Knop-Gericke, A. [Abteilung Anorganische Chemie, Fritz-Haber-Institut der Max-Planck-Gesellschaft, Faradayweg 4-6, D-14195 Berlin (Germany); Guo, J. H. [Advanced Light Source, Lawrence Berkeley National Laboratory, Berkeley, California 94720 (United States); Duda, L. C. [Department of Physics and Astronomy, Division of Molecular and Condensed Matter Physics, Uppsala University, Box 516, S-751 20 Uppsala (Sweden)

    2013-11-15

    We present a novel in situ reaction cell for heterogeneous catalysis monitored in situ by x-ray absorption spectroscopy (XAS) and resonant inelastic x-ray scattering (RIXS). The reaction can be carried out at a total pressure up to 1 atm, a regime that has not been accessible to comparable in situ techniques and thus closes the pressure gap to many industrial standard conditions. Two alternate catalyst geometries were tested: (A) a thin film evaporated directly onto an x-ray transparent membrane with a flowing reaction gas mixture behind it or (B) a powder placed behind both the membrane and a gap of flowing reaction gas mixture. To illustrate the working principle and feasibility of our reaction cell setup we have chosen ethylene epoxidation over a silver catalyst as a test case. The evolution of incorporated oxygen species was monitored by total electron/fluorescence yield O K-XAS as well as O K-RIXS, which is a powerful method to separate contributions from inequivalent sites. We find that our method can reliably detect transient species that exist during catalytic reaction conditions that are hardly accessible using other spectroscopic methods.

  15. Unusual Pulsed X-Ray Emission from the Young, High Magnetic Field Pulsar PSR J1119--6127

    Energy Technology Data Exchange (ETDEWEB)

    Gonzalez, M E; Kaspi, V M; Camilo, F; Gaensler, B M; Pivovaroff, M J

    2005-08-05

    We present XMM-Newton observations of the radio pulsar PSR J1119-6127, which has an inferred age of 1,700 yr and surface dipole magnetic field strength of 4.1 x 10{sup 13} G. We report the first detection of pulsed X-ray emission from PSR J1119-6127. In the 0.5-2.0 keV range, the pulse profile shows a narrow peak with a very high pulsed fraction of (74 {+-} 14)%. In the 2.0-10.0 keV range, the upper limit for the pulsed fraction is 28% (99% confidence). The pulsed emission is well described by a thermal blackbody model with a temperature of T{infinity} = 2.4{sub -0.2}{sup +0.3} x 10{sup 6} K and emitting radius of 3.4{sub -0.3}{sup +1.8} km (at a distance of 8.4 kpc). Atmospheric models result in problematic estimates for the distance/emitting area. PSR J1119-6127 is now the radio pulsar with smallest characteristic age from which thermal X-ray emission has been detected. The combined temporal and spectral characteristics of this emission are unlike those of other radio pulsars detected at X-ray energies and challenge current models of thermal emission from neutron stars.

  16. Crystallographic origin of perpendicular magnetic anisotropy in CoPt film: polarized x-ray absorption study

    Energy Technology Data Exchange (ETDEWEB)

    Pandey, K.K.M.; Chen, J.S.; Liu, T.; Sun, C.J.; Chow, G.M.; (NU Sinapore); (ORNL)

    2009-09-17

    Crystallographic structure, growth induced miscibility gap and strain in Ta/Co{sub 100-x}Pt{sub x} (0 {le} x {le} 43 at%)/Ru/Ta/glass films deposited at ambient temperature were investigated using polarized x-ray absorption spectroscopy to clarify the origin of observed perpendicular magnetic anisotropy (PMA) in Co{sub 72}Pt{sub 28} film. Extended x-ray absorption fine structure spectroscopy data at Co K-edge showed that Co has a similar local atomic environment and averaged interatomic distance in the in-plane and out-of-plane polarization geometries for Co{sub 72}Pt{sub 28}, ruling out the contribution of magneto-elastic anisotropy and growth induced structural anisotropy as the origin of PMA. A large PMA in Co{sub 72}Pt{sub 28} film was attributed to the preferred hexagonal close-packed stacking as observed using the x-ray absorption near-edge structure spectroscopy.

  17. Children's (Pediatric) Magnetic Resonance Imaging

    Medline Plus

    Full Text Available ... scanner. top of page How does the procedure work? Unlike conventional x-ray examinations and computed tomography ( ... as long as they are also screened for safety in the magnetic environment. Children will be given ...

  18. Magnetic Resonance Imaging (MRI) -- Head

    Medline Plus

    Full Text Available ... scanner. top of page How does the procedure work? Unlike conventional x-ray examinations and computed tomography ( ... as long as they are also screened for safety in the magnetic environment. Children will be given ...

  19. Magnetic Resonance Imaging (MRI) -- Head

    Medline Plus

    Full Text Available ... x-ray contrast material, drugs, food, or the environment, or if you have asthma. The contrast material ... are also screened for safety in the magnetic environment. Children will be given appropriately sized earplugs or ...

  20. Children's (Pediatric) Magnetic Resonance Imaging

    Medline Plus

    Full Text Available ... x-ray contrast material, drugs, food, or the environment, or if your child has asthma. The contrast ... are also screened for safety in the magnetic environment. Children will be given appropriately sized earplugs or ...

  1. Evidence for resonance electron transfer in photon excited X-ray satellite spectra of fluorine compounds

    Indian Academy of Sciences (India)

    K Ram Narayana; B Seetharami Reddy; S S Raju; T Seshi Reddy; S Lakshmi Narayana; K Premachand; B M Rao; M V R Murti; L S Mombasawala

    2005-08-01

    The KL1/KL0 intensity ratio of fluorine is measured in five fluorine compounds with a crystal spectrometer. An anomalous reduction of this intensity ratio was observed in KF and SrF2, which is attributed to resonance electron transfer from the metal ion to the spectator vacancy in the fluorine ion. KL2/KL0 intensity ratio of fluorine is also measured. The measured relative intensities are compared with the theoretical estimates of Aberg.

  2. X-ray magnetic circular dichroism and small angle neutron scattering study of thiol capped gold nanoparticles.

    Energy Technology Data Exchange (ETDEWEB)

    de la Venta, J.; Bouzas, V.; Pucci, A.; Laguna-Marco, M. A.; Haskel, D.; Pinel, E. F.; te Velthuis, S. G. E.; Hoffmann, A.; Lal, J.; Bleuel, M.; Ruggeri, G.; de Julian, C.; Garcia, M. A.; Univ. Complutense de Madrid; Inst. de Magnetismo Aplicado UCM; Univ. Pisa; Univ. di Padova

    2009-11-01

    X-ray magnetic circular dichroism (XMCD) and Small Angle Neutron Scattering (SANS) measurements were performed on thiol capped Au nanoparticles (NPs) embedded into polyethylene. An XMCD signal of 0.8 {center_dot} 10{sup -4} was found at the Au L{sub 3} edge of thiol capped Au NPs embedded in a polyethylene matrix for which Superconducting Quantum Interference Device (SQUID) magnetometry yielded a saturation magnetization, M{sub s}, of 0.06 emu/g{sub Au}. SANS measurements showed that the 3.2 nm average-diameter nanoparticles are 28% polydispersed, but no detectable SANS magnetic signal was found with the resolution and sensitivity accessible with the neutron experiment. A comparison with previous experiments carried out on Au NPs and multilayers, yield to different values between XMCD signals and magnetization measured by SQUID magnetometer. We discuss the origin of those differences.

  3. X-ray magnetic circular dichroism and small angle neutron scattering studies of thiol capped gold nanoparticles.

    Energy Technology Data Exchange (ETDEWEB)

    de la Venta, J.; Bouzas, V.; Pucci, A.; Laguna-Marco, M. A.; Haskel, D.; te Velthuis, S. G. E; Hoffmann, A.; Lal, J.; Bleuel, M.; Ruggeri, G.; de Julian Fernandez, C.; Garcia, M. A.; Univ.Complutense de Madrid; Inst. de Magnetismo Aplicado; Univ. of Pisa; Lab. di Magnetismo Molecolare

    2009-01-01

    X-ray magnetic circular dichroism (XMCD) and Small Angle Neutron Scattering (SANS) measurements were performed on thiol capped Au nanoparticles (NPs) embedded into polyethylene. An XMCD signal of 0.8 {center_dot} 10{sup -4} was found at the Au L{sub 3} edge of thiol capped Au NPs embedded in a polyethylene matrix for which Superconducting Quantum Interference Device (SQUID) magnetometry yielded a saturation magnetization, M{sub s}, of 0.06 emu/g{sub Au}. SANS measurements showed that the 3.2 nm average-diameter nanoparticles are 28% polydispersed, but no detectable SANS magnetic signal was found with the resolution and sensitivity accessible with the neutron experiment. A comparison with previous experiments carried out on Au NPs and multilayers, yield to different values between XMCD signals and magnetization measured by SQUID magnetometer. We discuss the origin of those differences.

  4. Domain wall velocity measurement in permalloy nanowires with X-ray magnetic circular dichroism imaging and single shot Kerr microscopy

    Energy Technology Data Exchange (ETDEWEB)

    Moore, T.A., E-mail: t.a.moore@physics.or [Fachbereich Physik, Universitaet Konstanz, Universitaetsstrasse 10, 78457 Konstanz (Germany); Klaeui, M.; Heyne, L.; Moehrke, P. [Fachbereich Physik, Universitaet Konstanz, Universitaetsstrasse 10, 78457 Konstanz (Germany); Backes, D.; Rhensius, J. [Fachbereich Physik, Universitaet Konstanz, Universitaetsstrasse 10, 78457 Konstanz (Germany); Laboratory for Micro- and Nanotechnology, Paul Scherrer Institut, 5232 Villigen PSI (Switzerland); Ruediger, U. [Fachbereich Physik, Universitaet Konstanz, Universitaetsstrasse 10, 78457 Konstanz (Germany); Heyderman, L.J. [Laboratory for Micro- and Nanotechnology, Paul Scherrer Institut, 5232 Villigen PSI (Switzerland); Mentes, T.O.; Nino, M.A.; Locatelli, A. [Sincrotrone Trieste, 34012 Basovizza-Trieste (Italy); Potenza, A.; Marchetto, H.; Cavill, S.; Dhesi, S.S. [Diamond Light Source Ltd., Harwell Science and Innovation Campus, Didcot, Oxfordshire, OX11 0DE (United Kingdom)

    2010-05-15

    Domain walls (DWs) propagated along nanoscale magnetic wires by current or field pulses could potentially be used for data storage or logic applications, but the understanding of the DW dynamics, particularly under the influence of spin-polarized current, is incomplete. Measuring the velocity can give insights into the physics of the DW motion. Here we demonstrate DW velocity measurements in permalloy (Ni{sub 80}Fe{sub 20}) nanowires (1500 nm width and 20 nm thickness) using the techniques of X-ray magnetic circular dichroism photoemission electron microscopy (XMCD-PEEM) to image the magnetic contrast in the nanowires, and single shot Kerr microscopy, which allows for dynamic measurements. The magnetic imaging yields the average velocity as well as information on the DW spin structure, whereas the single shot method highlights the stochastic nature of the DW motion.

  5. Stochastic limits in synchronous imaging of sub-micron magnetization dynamics using scanning transmission x-ray microscopy

    Energy Technology Data Exchange (ETDEWEB)

    Cheng C.; Kaznatcheev K.; Bailey, W.E.

    2012-02-28

    We demonstrate a synchronous (lock-in) technique for imaging thin-film magnetization dynamics using scanning transmission x-ray microscopy (STXM). Gated photon counting synchronized with magnetic field modulation allows image acquisition with differential contrast for high and low magnetization. We have applied this technique to 5 x 12 {micro}m{sup 2} Ni{sub 81}Fe{sub 19} ellipses with well-defined closure domains at remanence. The stochastic nature of the domain wall motion and nucleation is apparent in images recorded during cycling along successive major hysteresis loops. Synchronous imaging shows the clearest enhancement of contrast for small-amplitude domain wall motion, with a less obvious benefit at higher fields/displacements. The technique shows promise for the contrast enhancement of magnetization in dynamics in STXM.

  6. Skull x-ray

    Science.gov (United States)

    X-ray - head; X-ray - skull; Skull radiography; Head x-ray ... There is low radiation exposure. X-rays are monitored and regulated to provide the minimum amount of radiation exposure needed to produce the image. Most ...

  7. Neck x-ray

    Science.gov (United States)

    X-ray - neck; Cervical spine x-ray; Lateral neck x-ray ... There is low radiation exposure. X-rays are monitored so that the lowest amount of radiation is used to produce the image. Pregnant women and ...

  8. X-RAY POLARIZATION FROM HIGH-MASS X-RAY BINARIES

    Energy Technology Data Exchange (ETDEWEB)

    Kallman, T. [NASA/GSFC, Code 662, Greenbelt, MD 20771 (United States); Dorodnitsyn, A. [Department of Astronomy, University of Maryland, College Park, MD 20742 (United States); Blondin, J. [Department of Physics, North Carolina State University, Raleigh, NC 27695-8202 (United States)

    2015-12-10

    X-ray astronomy allows study of objects that may be associated with compact objects, i.e., neutron stars or black holes, and also may contain strong magnetic fields. Such objects are categorically nonspherical, and likely noncircular when projected on the sky. Polarization allows study of such geometric effects, and X-ray polarimetry is likely to become feasible for a significant number of sources in the future. Potential targets for future X-ray polarization observations are the high-mass X-ray binaries (HMXBs), which consist of a compact object in orbit with an early-type star. In this paper we show that X-ray polarization from HMXBs has a distinct signature that depends on the source inclination and orbital phase. The presence of the X-ray source displaced from the star creates linear polarization even if the primary wind is spherically symmetric whenever the system is viewed away from conjunction. Direct X-rays dilute this polarization whenever the X-ray source is not eclipsed; at mid-eclipse the net polarization is expected to be small or zero if the wind is circularly symmetric around the line of centers. Resonance line scattering increases the scattering fraction, often by large factors, over the energy band spanned by resonance lines. Real winds are not expected to be spherically symmetric, or circularly symmetric around the line of centers, owing to the combined effects of the compact object gravity and ionization on the wind hydrodynamics. A sample calculation shows that this creates polarization fractions ranging up to tens of percent at mid-eclipse.

  9. Induced magnetic anisotropy in Si-free nanocrystalline soft magnetic materials: A transmission x-ray diffraction study

    Energy Technology Data Exchange (ETDEWEB)

    Parsons, R., E-mail: rparsons01@gmail.com; Suzuki, K. [Department of Materials Science and Engineering, Monash University, Clayton, Victoria 3800 (Australia); Yanai, T. [Graduate School of Engineering, Nagasaki University, Nagasaki 852-8521 (Japan); Kishimoto, H.; Kato, A. [Toyota Motor Corporation, Mishuku, Susono, Shizuoka 410-1193 (Japan); Ohnuma, M. [Faculty and Graduate School of Engineering, Hokkaido University, Sapporo 060-8628 (Japan)

    2015-05-07

    In order to better understand the origin of field-induced anisotropy (K{sub u}) in Si-free nanocrystalline soft magnetic alloys, the lattice spacing of the bcc-Fe phase in nanocrystalline Fe{sub 94−x}Nb{sub 6}B{sub x} (x = 10, 12, 14) alloys annealed under an applied magnetic field has been investigated by X-ray diffraction in transmission geometry (t-XRD) with the diffraction vector parallel and perpendicular to the field direction. The saturation magnetostriction (λ{sub s}) of nanocrystalline Fe{sub 94−x}Nb{sub 6}B{sub x} was found to increase linearly with the volume fraction of the residual amorphous phase and is well described by taking into account the volume-weighted average of two local λ{sub s} values for the bcc-Fe nanocrystallites (−5 ± 2 ppm) and the residual amorphous matrix (+8 ± 2 ppm). The lattice distortion required to produce the measured K{sub u} values (∼100 J/m{sup 3}) was estimated via the inverse magnetostrictive effect using the measured λ{sub s} values and was compared to the lattice spacing estimations made by t-XRD. The lattice strain required to produce K{sub u} under the magnetoelastic model was not observed by the t-XRD experiments and so the findings of this study suggest that the origin of magnetic field induced K{sub u} cannot be explained through the magnetoelastic effect.

  10. Measurement of the polarization for soft x-ray magnetic circular dichroism at the BSRF beamline 4B7B

    CERN Document Server

    Zhi-Ying, Guo; Jing-Tao, Zhu; YI-Dong, Zhao; Lei, Zheng; Cai-Hao, Hong; Kun, Tang; Dong-Liang, Yang; Ming-Qi, Cui

    2012-01-01

    Three ultra-short-period W/B4C multilayers (1.244nm, 1.235nm and 1.034nm) have been fabricated and used for polarization measurement at the 4B7B Beamline of Beijing Synchrotron Radiation Facility (BSRF). By rotating analyzer ellipsometry method, the linear polarization degree of light emerging from this beamline has been measured and the circular polarization evaluated for 700eV-860eV. The first soft x-ray magnetic circular dichroism measurements are carried out at BSRF by positioning the beamline aperture out of the plane of the electron storage ring.

  11. Flare onsets in hard and soft X-rays. [magnetic energy conversion in sun

    Science.gov (United States)

    Machado, Marcos E.; Orwig, Larry E.; Antonucci, Ester

    1986-01-01

    It is shown that the onset of solar flares, within about 2 min or less before the impulsive peaks, is characterized by an increase in high-energy emission at E less than 100 keV, and strong broadening of soft X-ray lines characteristic of the 10-million-K plasma already present at this stage. The observations are interpreted in terms of the early signature of energy release, during a phase preceding the instability that leads to strong particle acceleration.

  12. Magnetic anisotropy in Ta/CoFeB/MgO investigated by x-ray magnetic circular dichroism and first-principles calculation

    Energy Technology Data Exchange (ETDEWEB)

    Kanai, Shun [Laboratory for Nanoelectronics and Spintronics, Research Institute of Electrical Communication, Tohoku University, 2-1-1 Katahira, Aoba-ku, Sendai 980-8577 (Japan); Tsujikawa, Masahito; Shirai, Masafumi [Center for Spintronics Integrated Systems, Tohoku University, 2-1-1 Katahira, Aoba-ku, Sendai 980-8577 (Japan); Research Institute of Electrical Communication, Tohoku University, 2-1-1 Katahira, Aoba-ku, Sendai 980-8577 (Japan); Miura, Yoshio [Research Institute of Electrical Communication, Tohoku University, 2-1-1 Katahira, Aoba-ku, Sendai 980-8577 (Japan); Department of Electronics and Information Science, Kyoto Institute of Technology, Kyoto (Japan); Matsukura, Fumihiro, E-mail: f-matsu@wpi-aimr.tohoku.ac.jp; Ohno, Hideo [Laboratory for Nanoelectronics and Spintronics, Research Institute of Electrical Communication, Tohoku University, 2-1-1 Katahira, Aoba-ku, Sendai 980-8577 (Japan); Research Institute of Electrical Communication, Tohoku University, 2-1-1 Katahira, Aoba-ku, Sendai 980-8577 (Japan); WPI-Advanced Institute for Materials Research (WPI-AIMR), Tohoku University, 2-1-1 Katahira, Aoba-ku, Sendai 980-8577 (Japan)

    2014-12-01

    We study the spin and orbital magnetic moments in Ta/Co{sub 0.4}Fe{sub 0.4}B{sub 0.2}/MgO by x-ray magnetic circular dichroism measurements as well as first-principles calculations, in order to clarify the origin of the perpendicular magnetic anisotropy. Both experimental and theoretical results show that orbital magnetic moment of Fe is more anisotropic than that of Co with respect to the magnetization direction. The anisotropy is larger for thinner CoFeB, indicating that Fe atoms at the interface with MgO contribute more than Co to the observed perpendicular magnetic anisotropy.

  13. Perpendicular magnetic anisotropy at the interface between ultrathin Fe film and MgO studied by angular-dependent x-ray magnetic circular dichroism

    Energy Technology Data Exchange (ETDEWEB)

    Okabayashi, J. [Research Center for Spectrochemistry, The University of Tokyo, Bunkyo-ku, Tokyo 113-0033 (Japan); Koo, J. W.; Mitani, S. [National Institute for Materials Science (NIMS), Tsukuba 305-0047 (Japan); Graduate School of Pure and Applied Sciences, University of Tsukuba, Tsukuba 305-8577 (Japan); Sukegawa, H. [National Institute for Materials Science (NIMS), Tsukuba 305-0047 (Japan); Takagi, Y.; Yokoyama, T. [Institute of Molecular Science, Okazaki, Aichi 444-8585 (Japan)

    2014-09-22

    Interface perpendicular magnetic anisotropy (PMA) in ultrathin Fe/MgO (001) has been investigated using angular-dependent x-ray magnetic circular dichroism (XMCD). We found that anisotropic orbital magnetic moments deduced from the analysis of XMCD contribute to the large PMA energies, whose values depend on the annealing temperature. The large PMA energies determined from magnetization measurements are related to those estimated from the XMCD and the anisotropic orbital magnetic moments through the spin-orbit interaction. The enhancement of anisotropic orbital magnetic moments can be explained mainly by the hybridization between the Fe 3d{sub z}{sup 2} and O 2p{sub z} states.

  14. Magnetically driven winds from differentially rotating neutron stars and X-ray afterglows of short gamma-ray bursts

    CERN Document Server

    Siegel, Daniel M; Rezzolla, Luciano

    2014-01-01

    Besides being among the most promising sources of gravitational waves, merging neutron-star binaries also represent a leading scenario to explain the phenomenology of short gamma-ray bursts (SGRBs). Recent observations have revealed a large subclass of SGRBs with roughly constant luminosity in their X-ray afterglows lasting 10-10^4 s. These features are generally taken as evidence for a long-lived central engine powered by the magnetic spin-down of a uniformly rotating magnetized object. We propose a different scenario in which the central engine powering the X-ray emission is a differentially rotating hypermassive neutron star (HMNS) that launches a quasi-isotropic and baryon-loaded wind driven by the magnetic field built-up through differential rotation. Our model is supported by long-term, three-dimensional, general-relativistic and ideal magnetohydrodynamic simulations showing that this isotropic emission is a very robust feature. For a given HMNS, the presence of a collimated component depends sensitivel...

  15. X-ray magnetic spectroscopy of MBE-grown Mn-doped Bi2Se3 thin films

    Directory of Open Access Journals (Sweden)

    L. J. Collins-McIntyre

    2014-12-01

    Full Text Available We report the growth of Mn-doped Bi2Se3 thin films by molecular beam epitaxy (MBE, investigated by x-ray diffraction (XRD, atomic force microscopy (AFM, SQUID magnetometry and x-ray magnetic circular dichroism (XMCD. Epitaxial films were deposited on c-plane sapphire substrates by co-evaporation. The films exhibit a spiral growth mechanism typical of this material class, as revealed by AFM. The XRD measurements demonstrate a good crystalline structure which is retained upon doping up to ∼7.5 atomic-% Mn, determined by Rutherford backscattering spectrometry (RBS, and show no evidence of the formation of parasitic phases. However an increasing interstitial incorporation of Mn is observed with increasing doping concentration. A magnetic moment of 5.1 μB/Mn is obtained from bulk-sensitive SQUID measurements, and a much lower moment of 1.6 μB/Mn from surface-sensitive XMCD. At ∼2.5 K, XMCD at the Mn L2,3 edge, reveals short-range magnetic order in the films and indicates ferromagnetic order below 1.5 K.

  16. Resonant X-ray emission spectroscopy reveals d-d ligand-field states involved in the self-assembly of a square-planar platinum complex.

    Science.gov (United States)

    Garino, Claudio; Gallo, Erik; Smolentsev, Nikolay; Glatzel, Pieter; Gobetto, Roberto; Lamberti, Carlo; Sadler, Peter J; Salassa, Luca

    2012-11-28

    Resonant X-ray Emission Spectroscopy (RXES) is used to characterize the ligand field states of the prototypic self-assembled square-planar complex, [Pt(tpy)Cl]Cl (tpy=2,2':6',2''-terpyridine), and determine the effect of weak metal-metal and π-π interactions on their energy.

  17. Discovery of a 112 ms X-Ray Pulsar in Puppis A: Further Evidence of Neutron Stars Weakly Magnetized at Birth

    Science.gov (United States)

    Gotthelf, E. V.; Halpern, J. P.

    2009-04-01

    We report the discovery of 112 ms X-ray pulsations from RX J0822-4300, the compact central object (CCO) in the supernova remnant (SNR) Puppis A, in two archival Newton X-Ray Multi-Mirror Mission observations taken in 2001. The sinusoidal light curve has a pulsed fraction of 11% with an abrupt 180° change in phase at 1.2 keV. The observed phase shift and modulation are likely the result of emission from opposing thermal hot spots of distinct temperatures. Phase-resolved spectra reveal an emission feature at E line = 0.8 keV associated with the cooler region, possibly due to an electron cyclotron resonance effect similar to that seen in the spectrum of the CCO pulsar 1E 1207.4-5209. No change in the spin period of PSR J0821-4300 is detected in seven months, with a 2σ upper limit on the period derivative of \\dot{P} Bs 220 kyr. The latter is much longer than the SNR age, indicating that PSR J0821-4300 was born spinning near its present period. Its properties are remarkably similar to those of the two other known CCO pulsars, demonstrating the existence of a class of neutron stars born with weak magnetic fields related to a slow original spin. These results are also of importance in understanding the extreme transverse velocity of PSR J0821-4300, favoring the hydrodynamic instability mechanism in the supernova explosion.

  18. Absorption lines from magnetically-driven winds in X-ray binaries

    CERN Document Server

    Chakravorty, S; Ferreira, J; Henri, G; Belmont, R; Clavel, M; Corbel, S; Rodriguez, J; Coriat, M; Drappeau, S; Malzac, J

    2016-01-01

    High resolution X-ray spectra of black hole X-ray binaries (BHBs) show blueshifted absorption lines from disk winds which seem to be equatorial. Winds occur in the Softer (disk-dominated) states of the outburst and are less prominent or absent in the Harder (power-law dominated) states. We use self-similar magneto-hydrodynamic (MHD) accretion-ejection models to explain the disk winds in BHBs. In our models, the density at the base of the outflow from the accretion disk is not a free parameter, but is determined by solving the full set of dynamical MHD equations. Thus the physical properties of the outflow are controlled by the global structure of the disk. We studied different MHD solutions characterized by different values of (a) the disk aspect ratio ($\\varepsilon$) and (b) the ejection efficiency ($p$). We use two kinds of MHD solutions depending on the absence (cold solution) or presence (warm solution) of heating at the disk surface. Such heating could be from e.g. dissipation of energy due to MHD turbul...

  19. A Study of the X-Ray Emission of Magnetic Cataclysmic Variable Ae Aquarii

    CERN Document Server

    Choi, C S; Agrawal, P C; Choi, Chul-Sung; Dotani, Tadayasu

    1999-01-01

    We report results from analysis of the X-ray observations of AE Aqr, made with Ginga in June 1988 and with ASCA in October 1995. Pulsations are detected clearly with a sinusoidal pulse profile with periods of $33.076\\pm0.001$ s (Ginga) and $33.077\\pm0.003$ s (ASCA)\\@. The pulse amplitude is relatively small and the modulated flux remains nearly constant despite a factor of 3 change in the average flux during the flare. We reproduce the time-averaged spectrum in the 0.4 -- 10 keV energy band by a thermal emission model with a combination of two different temperatures: kT$_1 = 0.68^{+0.01}_{-0.02}$ keV and kT$_2 = 2.9^{+0.3}_{-0.2}$ keV\\@. There is no significant difference between the quiescent and flare energy spectra, although a hint of spectral hardening is recognized during the flare. We interpret these observational results with a model in which AE Aqr is in a propeller stage. Based on this propeller scenario, we suggest that the X-ray emission is originated from magnetospheric radiation.

  20. Demonstration of the self-magnetic-pinch diode as an X-ray source for flash core-punch radiography.

    Energy Technology Data Exchange (ETDEWEB)

    Cordova, Steve Ray; Rovang, Dean Curtis; Portillo, Salvador; Oliver, Bryan Velten; Bruner, Nichelle Lee (Voss Scientific, Albuquerque, NM); Ziska, Derek Raymond (K-Tech Corporation, Albuquerque, NM)

    2007-10-01

    Minimization of the radiographic spot size and maximization of the radiation dose is a continuing long-range goal for development of electron beam driven X-ray radiography sources. In collaboration with members of the Atomic Weapons Establishment(AWE), Aldermaston UK, the Advanced Radiographic Technologies Dept. 1645 is conducting research on the development of X-ray sources for flash core-punch radiography. The Hydrodynamics Dept. at AWE has defined a near term radiographic source requirement for scaled core-punch experiments to be 250 rads{at}m with a 2.75 mm source spot-size. As part of this collaborative effort, Dept. 1645 is investigating the potential of the Self-Magnetic-Pinched (SMP) diode as a source for core-punch radiography. Recent experiments conducted on the RITS-6 accelerator [1,2] demonstrated the potential of the SMP diode by meeting and exceeding the near term radiographic requirements established by AWE. During the demonstration experiments, RITS-6 was configured with a low-impedance (40 {Omega}) Magnetically Insulated Transmission Line (MITL), which provided a 75-ns, 180-kA, 7.5-MeV forward going electrical pulse to the diode. The use of a low-impedance MITL enabled greater power coupling to the SMP diode and thus allowed for increased radiation output. In addition to reconfiguring the driver (accelerator), geometric changes to the diode were also performed which allowed for an increase in dose production without sacrificing the time integrated spot characteristics. The combination of changes to both the pulsed power driver and the diode significantly increased the source x-ray intensity.

  1. X-ray magnetic and natural circular dichroism from first principles: Calculation of K - and L1-edge spectra

    Science.gov (United States)

    Bouldi, N.; Vollmers, N. J.; Delpy-Laplanche, C. G.; Joly, Y.; Juhin, A.; Sainctavit, Ph.; Brouder, Ch.; Calandra, M.; Paulatto, L.; Mauri, F.; Gerstmann, U.

    2017-08-01

    An efficient first-principles approach to calculate x-ray magnetic circular dichroism (XMCD) and x-ray natural circular dichroism (XNCD) is developed and applied in the near-edge region at the K and L1 edges in solids. Computation of circular dichroism requires precise calculations of x-ray absorption spectra (XAS) for circularly polarized light. For the derivation of the XAS cross section, we used a relativistic description of the photon-electron interaction that results in an additional term in the cross section that couples the electric dipole operator with an operator σ .(ɛ ×r ) that we call the spin position operator. The numerical method relies on pseudopotentials, on the gauge including projected augmented-wave method, and on a collinear spin relativistic description of the electronic structure. We apply the method to calculations of K -edge XMCD spectra of ferromagnetic iron, cobalt, and nickel and of I L1-edge XNCD spectra of α -LiIO3 , a compound with broken inversion symmetry. For XMCD spectra we find that, even if the electric dipole term is the dominant one, the electric quadrupole term is not negligible (8% in amplitude in the case of iron). The term coupling the electric dipole operator with the spin-position operator is significant (28% in amplitude in the case of iron). We obtain a sum rule relating this term to the spin magnetic moment of the p states. In α -LiIO3 we recover the expected angular dependence of the XNCD spectra.

  2. Detection of cyclotron resonance scattering feature in high-mass X-ray binary pulsar SMC X-2

    Science.gov (United States)

    Jaisawal, Gaurava K.; Naik, Sachindra

    2016-09-01

    We report broad-band spectral properties of the high-mass X-ray binary pulsar SMC X-2 by using three simultaneous Nuclear Spectroscopy Telescope Array and Swift/XRT observations during its 2015 outburst. The pulsar was significantly bright, reaching a luminosity up to as high as ˜5.5 × 1038 erg s-1 in 1-70 keV range. Spin period of the pulsar was estimated to be 2.37 s. Pulse profiles were found to be strongly luminosity dependent. The 1-70 keV energy spectrum of the pulsar was well described with three different continuum models such as (i) negative and positive power law with exponential cutoff, (ii) Fermi-Dirac cutoff power law and (iii) cutoff power-law models. Apart from the presence of an iron line at ˜6.4 keV, a model independent absorption like feature at ˜27 keV was detected in the pulsar spectrum. This feature was identified as a cyclotron absorption line and detected for the first time in this pulsar. Corresponding magnetic field of the neutron star was estimated to be ˜2.3 × 1012 G. The cyclotron line energy showed a marginal negative dependence on the luminosity. The cyclotron line parameters were found to be variable with pulse phase and interpreted as due to the effect of emission geometry or complicated structure of the pulsar magnetic field.

  3. Correcting and coating thin walled X-ray Optics via a combination of controlled film deposition and magnetic smart materials

    Science.gov (United States)

    Ulmer, Melville

    The project goal is to demonstrate that thin walled (price. Since the desired surface area for the next generation X-ray telescope is >10x that of Chandra, the >10x requirement is then for >200 m^2 of surface area with a surface finish of better than 0.5 nm. Therefore, replication of some sort is called for. Because no replication technology has been shown to achieve ≤1" angular resolution, post fabrication figure corrections are likely going to be necessary. Some have proposed to do this in orbit and others prelaunch including us. Our prelaunch approach is to apply in-plane stresses to the thin walled mirror shells via a magnetic field. The field will be held in by some magnetically hard material such as NiCo. By use of a so called magnetic smart material (MSM) such as Terfenol-D, we already shown that strong enough stresses can be generated. Preliminary work has also shown that the magnetic field can be held in well enough to apply the figure correcting stresses pre-launch. What we call "set-it and forget-it." However, what is unique about our approach is that at the cost of complexity and some areal coverage, our concept will also accommodate in-orbit adjustments. Furthermore, to the best of our knowledge ours is one of two known stress modification processes that are bi-axial. Our plan is first to validate set-it and forget-it first on cantilevers and then to expand this to working on 5 cm x 5 cm pieces. We will work both with NiCo and glass or Si coated with Terfenol-D. Except for the NiCo, substrates we will also coat the samples with NiCo in order to have a film that will hold in the magnetic field. As part of the coating process, we will control the stress of the film by varying the voltage bias while coating. The bias stress control can be used to apply films with minimal stress such as Terfenol-D and X-ray reflecting coatings such as Ir. Ir is a highly desirable coating for soft X-ray astronomy mirrors that can have significant built in stress unless

  4. The first observed stellar X-ray flare oscillation: Constraints on the flare loop length and the magnetic field

    CERN Document Server

    Mitra-Kraev, U; Williams, D R; Kraev, E

    2005-01-01

    We present the first X-ray observation of an oscillation during a stellar flare. The flare occurred on the active M-type dwarf AT Mic and was observed with XMM-Newton. The soft X-ray light curve (0.2-12 keV) is investigated with wavelet analysis. The flare's extended, flat peak shows clear evidence for a damped oscillation with a period of around 750 s, an exponential damping time of around 2000 s, and an initial, relative peak-to-peak amplitude of around 15%. We suggest that the oscillation is a standing magneto-acoustic wave tied to the flare loop, and find that the most likely interpretation is a longitudinal, slow-mode wave, with a resulting loop length of (2.5 +- 0.2) e10 cm. The local magnetic field strength is found to be (105 +- 50) G. These values are consistent with (oscillation-independent) flare cooling time models and pressure balance scaling laws. Such a flare oscillation provides an excellent opportunity to obtain coronal properties like the size of a flare loop or the local magnetic field stre...

  5. An electron spin double resonance study of x-ray irradiated phenacyl chloride single crystals

    Science.gov (United States)

    Hwang, J. S.; Wang, H. C.; Andersson, B.; Kispert, L. D.; Geoffroy, M.

    1981-10-01

    Single crystals of phenacyl chloride irradiated at room temperature give rise to an EPR spectrum that has been shown by ENDOR and ELDOR studies to be due to the radical The EPR spectra are complicated by the appearance of a large number of forbidden lines due to the presence of a chlorine quadrupole interaction similar in magnitude to the proton hyperfine coupling. Spectral assignment is not possible by considering the EPR spectra alone. Although ENDOR spectra are difficult to obtain, it is possible to obtain an ENDOR spectrum along one of the crystal axis that identifies the spectra as due to radical I. Furthermore, rather intense and highly resolved ELDOR spectra are obtained at -60 °C as a function of angle enabling the chlorine and proton magnetic hyperfine tensor components of the -ĊHCl fragment to be determined as -15.4, -8.3, +45.6 MHz and -26.5, -52.5, -80.0 MHz, respectively. The Qzz components of the chlorine quadrupole tensor is -11.2 MHz.

  6. Erbium-doped yttrium aluminum garnet as a magnetic refrigerant for low temperature x-ray detectors

    Science.gov (United States)

    Kushino, Akihiro; Aoki, Yuji; Yamasaki, Noriko Y.; Namiki, Takahiro; Ishisaki, Yoshitaka; Matsuda, Tatsuma D.; Ohashi, Takaya; Mitsuda, Kazuhisa; Yazawa, Takashi

    2001-12-01

    Garnets doped with rare-earth elements can be used in adiabatic demagnetization refrigerators. We have measured the specific heat and magnetization of a single crystal yttrium aluminum garnet (YAG) doped with 30% Er3+ ion at temperatures between 93 mK and 8 K under magnetic fields up to 8.0 T along the crystal axis. From the specific heat and magnetization, we derived consistent temperature and magnetic-field dependence of the magnetic entropy. Under zero magnetic field, the magnetic entropy begins to decrease below 2 K and becomes half of R ln 2 at ˜160 mK. This decrease is considered to be due to an antiferromagnetic short-range ordering among Er3+ ions. This behavior of the specific heat in the measured temperature range can be explained by a model in which both the crystalline-electric-field ground state and the first excited state are included. The operating temperature of the Er3+-doped YAG as a magnetic coolant is estimated to extend down to ˜100 mK, which is lower than those with nonsubstituted garnets such as gallium-gadolinium-garnet used in the range ˜4.2-15 K. With a doping level of 30%, we estimate that ˜6 kg of Er3+-doped YAG exhibits the same cooling performance at 60 mK as the 916 g of ferric-ammonium-alum salt used for the x-ray spectrometer (microcalorimeter detectors) on the Astro-E satellite.

  7. Extracting magnetic cluster size and its distributions in advanced perpendicular recording media with shrinking grain size using small angle x-ray scattering

    Energy Technology Data Exchange (ETDEWEB)

    Mehta, Virat; Ikeda, Yoshihiro; Takano, Ken; Terris, Bruce D.; Hellwig, Olav [San Jose Research Center, HGST a Western Digital company, 3403 Yerba Buena Rd., San Jose, California 95135 (United States); Wang, Tianhan [Department of Materials Science and Engineering, Stanford University, Stanford, California 94035 (United States); Stanford Institute for Materials and Energy Science (SIMES), SLAC National Accelerator Laboratory, 2575 Sand Hill Road, Menlo Park, California 94025 (United States); Wu, Benny; Graves, Catherine [Stanford Institute for Materials and Energy Science (SIMES), SLAC National Accelerator Laboratory, 2575 Sand Hill Road, Menlo Park, California 94025 (United States); Department of Applied Physics, Stanford University, Stanford, California 94035 (United States); Dürr, Hermann A.; Scherz, Andreas; Stöhr, Jo [Stanford Institute for Materials and Energy Science (SIMES), SLAC National Accelerator Laboratory, 2575 Sand Hill Road, Menlo Park, California 94025 (United States)

    2015-05-18

    We analyze the magnetic cluster size (MCS) and magnetic cluster size distribution (MCSD) in a variety of perpendicular magnetic recording (PMR) media designs using resonant small angle x-ray scattering at the Co L{sub 3} absorption edge. The different PMR media flavors considered here vary in grain size between 7.5 and 9.5 nm as well as in lateral inter-granular exchange strength, which is controlled via the segregant amount. While for high inter-granular exchange, the MCS increases rapidly for grain sizes below 8.5 nm, we show that for increased amount of segregant with less exchange the MCS remains relatively small, even for grain sizes of 7.5 and 8 nm. However, the MCSD still increases sharply when shrinking grains from 8 to 7.5 nm. We show evidence that recording performance such as signal-to-noise-ratio on the spin stand correlates well with the product of magnetic cluster size and magnetic cluster size distribution.

  8. Investigation of the electronic structure of CuO by means of resonant X-ray Raman scattering

    CERN Document Server

    Doering, G

    2001-01-01

    excited state. By means of a perturbation theoretical treatment of the Coulomb interaction between the core-hole and the 3d-electrons an expression for the cross-section of the shakeup-process is derived. Thereby the observed excitation energy dependence of the shakeup-satellite's intensity and its position in the energy loss spectrum can be explained. Furthermore, its intensity shows a strong dependence on the scattering angle in certain scattering geometries. By means of a model calculation this dependence is attributed to a polarisation-effect. In this thesis the electronic structure of CuO is investigated utilizing resonant X-ray Raman Scattering. The special properties of this transition metal oxide are emphasized and the potential of the method is shown. First it is explained how one can draw conclusions about the unoccupied density of states of CuO and its symmetry from measurements of the copper K-alpha fluorescence by using an excitation energy of a few eV below the absorption threshold. By this mean...

  9. Resonant soft X-ray reflectivity of ultrathin polymer films at the C-edge: A direct approach

    Directory of Open Access Journals (Sweden)

    Alain Gibaud

    2016-09-01

    Full Text Available The use of resonant soft X-ray reflectivity (RSXRR in s-polarization is presented with the aim to show how far it is possible to go in the understanding the evolution of the refractive index n(E=1−δ(E−iβ(E of a ultrathin polystyrene film when the RSXRR is measured through the C-edge. We evidence that a direct fit to the data provides a very good estimation of δ(E and β(E in a large range of energies. Nevertheless, at some specific energy close to C-edge we observe that it is not possible to obtain a satisfactory fit to the data though the same formalism is applied to calculate the reflectivity. We show that even though we take into account the energy resolution of the incident beam, we still end up with a poor fit at these energies. Incorporating the strong contribution of 2nd order photons appeared near C-edge we could not eliminate the discrepancy. Probably the data normalisations have some impacts on such discrepancies at some specific energies.

  10. Resonant soft X-ray reflectivity of ultrathin polymer films at the C-edge: A direct approach

    Science.gov (United States)

    Gibaud, Alain; Bal, Jayanta Kumar; Gullikson, Eric M.; Wang, Cheng; Vignaud, Guillaume

    2016-09-01

    The use of resonant soft X-ray reflectivity (RSXRR) in s-polarization is presented with the aim to show how far it is possible to go in the understanding the evolution of the refractive index n (E ) =1 -δ (E ) -i β (E ) of a ultrathin polystyrene film when the RSXRR is measured through the C-edge. We evidence that a direct fit to the data provides a very good estimation of δ (E ) and β (E ) in a large range of energies. Nevertheless, at some specific energy close to C-edge we observe that it is not possible to obtain a satisfactory fit to the data though the same formalism is applied to calculate the reflectivity. We show that even though we take into account the energy resolution of the incident beam, we still end up with a poor fit at these energies. Incorporating the strong contribution of 2nd order photons appeared near C-edge we could not eliminate the discrepancy. Probably the data normalisations have some impacts on such discrepancies at some specific energies.

  11. Detecting non-bridging oxygens: non-resonant inelastic X-ray scattering in crystalline lithium borates.

    Science.gov (United States)

    Lelong, Gérald; Radtke, Guillaume; Cormier, Laurent; Bricha, Hanane; Rueff, Jean-Pascal; Ablett, James M; Cabaret, Delphine; Gélébart, Frédéric; Shukla, Abhay

    2014-10-20

    Probing the local environment of low-Z elements, such as oxygen, is of great interest for understanding the atomic-scale behavior in materials, but it requires experimental techniques allowing it to work with versatile sample environments. In this paper, the local environment of lithium borate crystals is investigated using non-resonant inelastic X-ray scattering (NRIXS) at energy losses corresponding to the oxygen K-edge. Large variations of the spectral features are observed close to the edge onset in the 535-540 eV energy range when varying the Li2O content. Calculations allow identification of contributions associated with bridging oxygen (BO) and non-bridging oxygen (NBO) atoms. The main result resides in the observed core-level shift of about 1.7 eV in the spectral signatures of the BO and NBO. The clear signature at 535 eV in the O K-edge NRXIS spectrum is thus an original way to probe the presence of NBOs in borates, with the great advantage of making possible the use of complex environments such as a high-pressure cell or high-temperature device for in situ measurements.

  12. Experimental observation of temperature and magnetic-field evolution of the 4 f states in CeFe2 revealed by soft x-ray magnetic circular dichroism

    Science.gov (United States)

    Saitoh, Y.; Yasui, A.; Fuchimoto, H.; Nakatani, Y.; Fujiwara, H.; Imada, S.; Narumi, Y.; Kindo, K.; Takahashi, M.; Ebihara, T.; Sekiyama, A.

    2017-07-01

    We revisit the delocalized character of the 4 f states of CeFe2 in the ferromagnetically ordered phase by x-ray magnetic circular dichroism (XMCD) in x-ray absorption spectroscopy (XAS) with improved data quality using single crystals. Surprisingly, the Ce M4 ,5 XMCD spectral shape changes significantly as a function of temperature and applied magnetic field, with no concomitant changes in the spectral shape of the Ce M4 ,5 XAS as well as the Fe L2 ,3 XAS and XMCD. This unusual behavior is characterized by the J =7 /2 states in a 4 f1 configuration mixed into the J =5 /2 ground state. Such extreme sensitivity of the Ce 4 f states to the external perturbations can be related to the magnetic instability toward an antiferromagnetic phase in CeFe2. Our experimental data presented here provide valuable insights into the underlying physics in strongly hybridized ferromagnetic Ce compounds.

  13. Characterization of thin-film multilayers using magnetization curves and modeling of low-angle X-ray diffraction data

    Energy Technology Data Exchange (ETDEWEB)

    Lane, M. [Emory & Henry College, VA (United States); Chaiken, A.; Michel, R.P. [Lawrence Livermore National Lab., CA (United States)

    1994-12-01

    We have characterized thin-film multilayers grown by ion-beam sputtering using magnetization curves and modeling of low-angle x-ray diffraction data. In our films, we use ferromagnetic layer = Co, Fe, and NiFe and spacer layer = Si, Ge, FeSi{sub 2}, and CoSi{sub 2}. We have studied the effects of (1) deposition conditions; (2) thickness of layers; (3) different layer materials; and (4) annealing. We find higher magnetization in films grown at 1000V rather than 500V and in films with spacer layers of 50{angstrom} rather than 100{angstrom}. We find higher coercivity in films with cobalt grown on germanium rather than silicon, metal grown on gold underlayers rather than on glass substrates, and when using thinner spacer layers. Finally, modeling reveals that films grown with disilicide layers are more thermally stable than films grown with silicon spacer layers.

  14. Search for Two-Photon Interaction with Axionlike Particles Using High-Repetition Pulsed Magnets and Synchrotron X Rays

    Science.gov (United States)

    Inada, T.; Yamazaki, T.; Namba, T.; Asai, S.; Kobayashi, T.; Tamasaku, K.; Tanaka, Y.; Inubushi, Y.; Sawada, K.; Yabashi, M.; Ishikawa, T.; Matsuo, A.; Kawaguchi, K.; Kindo, K.; Nojiri, H.

    2017-02-01

    We report on new results of a search for a two-photon interaction with axionlike particles (ALPs). The experiment is carried out at a synchrotron radiation facility using a "light shining through a wall (LSW)" technique. For this purpose, we develop a novel pulsed-magnet system, composed of multiple racetrack magnets and a transportable power supply. It produces fields of about 10 T over 0.8 m with a high repetition rate of 0.2 Hz and yields a new method of probing a vacuum with high intensity fields. The data obtained with a total of 27 676 pulses provide a limit on the ALP-two-photon coupling constant that is more stringent by a factor of 5.2 compared to a previous x-ray LSW limit for the ALP mass ≲0.1 eV .

  15. Search for Two-Photon Interaction with Axionlike Particles Using High-Repetition Pulsed Magnets and Synchrotron X Rays

    CERN Document Server

    Inada, T; Namba, T; Asai, S; Kobayashi, T; Tamasaku, K; Tanaka, Y; Inubushi, Y; Sawada, K; Yabashi, M; Ishikawa, T; Matsuo, A; Kawaguchi, K; Kindo, K; Nojiri, H

    2016-01-01

    We report on new results of a search for two-photon interaction with axionlike particles (ALPs). The experiment was carried out at a synchrotron radiation facility using a "light shining through a wall (LSW)" technique. For this purpose, we have developed a novel pulsed-magnet system, composed of multiple racetrack-magnets and a transportable power supply. It produces fields of about 10 T over 0.8 m with a high repetition rate of 0.2 Hz and yields a new method of probing vacuum with high intensity fields. The data obtained with a total of 27,676 pulses provide a limit on the ALP-two-photon coupling constant that is more stringent by a factor of 5.2 compared to a previous x-ray LSW limit for the ALP mass below 0.1 eV.

  16. Neutron and X-ray single-crystal diffraction from protein microcrystals via magnetically oriented microcrystal arrays in gels.

    Science.gov (United States)

    Tsukui, Shu; Kimura, Fumiko; Kusaka, Katsuhiro; Baba, Seiki; Mizuno, Nobuhiro; Kimura, Tsunehisa

    2016-07-01

    Protein microcrystals magnetically aligned in D2O hydrogels were subjected to neutron diffraction measurements, and reflections were observed for the first time to a resolution of 3.4 Å from lysozyme microcrystals (∼10 × 10 × 50 µm). This result demonstrated the possibility that magnetically oriented microcrystals consolidated in D2O gels may provide a promising means to obtain single-crystal neutron diffraction from proteins that do not crystallize at the sizes required for neutron diffraction structure determination. In addition, lysozyme microcrystals aligned in H2O hydrogels allowed structure determination at a resolution of 1.76 Å at room temperature by X-ray diffraction. The use of gels has advantages since the microcrystals are measured under hydrated conditions.

  17. Precession of Magnetically Driven Warped Disks and Low-Frequency QPOs in Low-Mass X-Ray Binaries

    CERN Document Server

    Shirakawa, A; Shirakawa, Akiko; Lai, Dong

    2000-01-01

    An accretion disk around a rotating magnetized star is subjected to magnetic torques which induce disk warping and precession. These torques arise generically from interactions between the stellar field and the induced surface currents on the disk. Applying these new effects to weakly magnetized ($B\\sim$ $10^7$-$10^9$ G) neutron stars in low-mass X-ray binaries, we study the global hydrodynamical warping/precession modes of the disk under the combined influences of relativistic frame dragging and the magnetic torques. Under quite general conditions, the magnetic warping torque can overcome the ``Bardeen-Petterson'' viscous damping and makes the modes grow. The modes are confined to the inner region of the disk, and have frequencies close to the sum of the Lense-Thirring frequency and the magnetically driven precession frequency evaluated at the inner disk radius. Since the magnetically driven precession is retrograde (and opposite to the Lense-Thrring precession), the mode frequency can have a non-monotonic d...

  18. X-ray resonant photoexcitation: line widths and energies of K{\\alpha} transitions in highly charged Fe ions

    CERN Document Server

    Rudolph, J K; Epp, S W; Steinbrügge, R; Beilmann, C; Brown, G V; Eberle, S; Graf, A; Harman, Z; Hell, N; Leutenegger, M; Müller, A; Schlage, K; Wille, H -C; Yavas, H; Ullrich, J; López-Urrutia, J R Crespo

    2013-01-01

    Photoabsorption by and fluorescence of the K{\\alpha} transitions in highly charged iron ions are essential mechanisms for X-ray radiation transfer in astrophysical environments. We study photoabsorption due to the main K{\\alpha} transitions in highly charged iron ions from heliumlike to fluorinelike (Fe 24+...17+) using monochromatic X-rays around 6.6 keV at the PETRA III synchrotron photon source. Natural linewidths were determined with hitherto unattained accuracy. The observed transitions are of particular interest for the understanding of photoexcited plasmas found in X-ray binaries and active galactic nuclei.

  19. BIGEL analysis of gene expression in HL60 cells exposed to X rays or 60 Hz magnetic fields

    Science.gov (United States)

    Balcer-Kubiczek, E. K.; Zhang, X. F.; Han, L. H.; Harrison, G. H.; Davis, C. C.; Zhou, X. J.; Ioffe, V.; McCready, W. A.; Abraham, J. M.; Meltzer, S. J.

    1998-01-01

    We screened a panel of 1,920 randomly selected cDNAs to discover genes that are differentially expressed in HL60 cells exposed to 60 Hz magnetic fields (2 mT) or X rays (5 Gy) compared to unexposed cells. Identification of these clones was accomplished using our two-gel cDNA library screening method (BIGEL). Eighteen cDNAs differentially expressed in X-irradiated compared to control HL60 cells were recovered from a panel of 1,920 clones. Differential expression in experimental compared to control cells was confirmed independently by Northern blotting of paired total RNA samples hybridized to each of the 18 clone-specific cDNA probes. DNA sequencing revealed that 15 of the 18 cDNA clones produced matches with the database for genes related to cell growth, protein synthesis, energy metabolism, oxidative stress or apoptosis (including MYC, neuroleukin, copper zinc-dependent superoxide dismutase, TC4 RAS-like protein, peptide elongation factor 1alpha, BNIP3, GATA3, NF45, cytochrome c oxidase II and triosephosphate isomerase mRNAs). In contrast, BIGEL analysis of the same 1,920 cDNAs revealed no differences greater than 1.5-fold in expression levels in magnetic-field compared to sham-exposed cells. Magnetic-field-exposed and control samples were analyzed further for the presence of mRNA encoding X-ray-responsive genes by hybridization of the 18 specific cDNA probes to RNA from exposed and control HL60 cells. Our results suggest that differential gene expression is induced in approximately 1% of a random pool of cDNAs by ionizing radiation but not by 60 Hz magnetic fields under the present experimental conditions.

  20. Characterization of Biochar by X-Ray Photoelectron Spectroscopy and 13 C Nuclear Magnetic Resonance%X射线光电子能谱与13 C核磁共振在生物质碳表征中的应用

    Institute of Scientific and Technical Information of China (English)

    徐东昱; 金洁; 颜钰; 韩兰芳; 康明洁; 王子莹; 赵烨; 孙可

    2014-01-01

    近年来,生物质碳(biochar)作为新型吸附剂被广泛研究。但由于制备biochar的生物质原料和热解温度的不同,使biochar的结构和组成存在差异,从而影响其对污染物的吸附。目前关于biochar的结构和组成的研究还不够全面。因此,结合了能谱与光谱分析的手段,对biochar的结构和组成进行了深入的分析。选取木质类(柳树枝条)和草类(水稻秸秆)作为原料,分别在不同热解温度(300,450和600℃)下制得bio-chars,并对biochars样品进行元素分析、X射线光电子能谱分析(XPS)和固态13C核磁共振(13CNMR)研究,以阐明不同热解温度和生物质来源的biochars的结构和组成。结果显示:biochar的H/C,O/C和(O+N)/C的比值随着热解温度的升高而降低;草类biochar比木质类biochar具有更高的灰分含量和表面极性;木质类biochar的矿物主要分布在样品颗粒内部,其表面被有机质覆盖,而草类biochar部分矿物暴露在样品颗粒表面;13CNMR显示低温制得的biochar主要由芳香碳、脂肪碳、羧基和羰基碳组成,高温制得的biochar主要由芳香碳组成,且低温制得biochars中,木质类biochars比草类biochars含有更高的木质素的残留碳结构,这是由于木质类biochars原材料中含有更高的木质素。%The wood (willow branch) and grass (rice straw ) materials were pyrolyzed at different temperatures (300 ,450 and 600 ℃) to obtain the biochars used in the present study .The biochars were characterized using elementary analysis ,X-ray pho-toelectron spectroscopy (XPS) and solid state 13 C cross-polarization and magic angle spinning nuclear magnetic resonance spec-troscopy (13C NMR) to illuminate the structure and composition of the biochars which were derived from the different thermal temperatures and biomass .The results showed that the H/C ,O/C and (O+N)/C ratios of the biochars decreased with

  1. X-ray and H-alpha observations of a filament-disappearance flare - An empirical analysis of the magnetic field configuration

    Science.gov (United States)

    Kahler, S. W.; Webb, D. F.; Moore, R. L.

    1981-01-01

    On August, 29, 1973, a flare event occurred that involved the disappearance of a filament near central meridian. The event, well-observed in X-rays on Skylab and in H-alpha, was a four-ribbon flare involving both new and old magnetic inversion lines which were roughly parallel. The H-alpha, X-ray, and magnetic field data are used to deduce the magnetic polarities of the H-alpha brightening at the footpoints of the brightest X-ray loops. It is suggested that the event involved a reconnection of magnetic field lines rather than a brightening in place of preexisting loops. The simultaneity of the H-alpha brightening onsets in the four ribbons and the apparent lack of an eruption of the filament are consistent with this interpretation.

  2. X-ray Hotspot Flares and Implications for Cosmic Ray Acceleration and Magnetic Field amplification in Supernova Remnants

    CERN Document Server

    Butt, Yousaf; Katz, Boaz; Waxman, Eli

    2008-01-01

    For more than fifty years, it has been believed that cosmic ray (CR) nuclei are accelerated to high energies in the rapidly expanding shockwaves created by powerful supernova explosions. Yet observational proof of this conjecture is still lacking. Recently, Uchiyama and collaborators reported the detection of small-scale X-ray flares in one such supernova remnant, dubbed 'RX J1713-3946' (a.k.a. G347.3-0.5), which also emits very energetic, TeV (10^12 eV) range, gamma-rays. They contend that the variability of these X-ray 'hotspots' implies that the magnetic field in the remnant is about a hundred times larger than normally assumed; and this, they say, means that the detected TeV range photons were produced in energetic nuclear interactions, providing 'a strong argument for acceleration of protons and nuclei to energies of 1 PeV (10^15 eV) and beyond in young supernova remnants.' We point out here that the existing multiwavelength data on this object certainly do not support such conclusions. Though intriguing...

  3. Predictions for Fourier-resolved X-ray spectroscopy from the model of magnetic flare avalanches above an accretion disc with hot ionized skin

    CERN Document Server

    Zycki, P T

    2002-01-01

    The magnetic flare avalanches model of Poutanen & Fabian for X-ray variability of accreting black holes is combined with computations of vertical structure of illuminated accretion discs in hydrostatic equilibrium. The latter predict the existence of a hot ionized skin, due to the thermal instability of X-ray illuminated plasma. The presence of such ionized skin, with properties dependent on disc radius, introduces a dependence of the emitted X-ray spectrum on the position on the disc. If the position is related to the time scale of the flares, the X-ray energy spectra (both the primary continuum and the reprocessed component) gain an additional dependence on Fourier frequency, beside that resulting from spectral evolution during a flare. We compute the Fourier frequency resolved spectra in this model and demonstrate that the presence of the hot skin introduces trends opposite to those observed in black hole binaries. Furthermore, the flare profile is strongly constrained, if the Fourier frequency depende...

  4. Structural and magnetic properties of transition metal substituted BaFe2As2 compounds studied by x-ray and neutron scattering

    Energy Technology Data Exchange (ETDEWEB)

    Kim, Min Gyu [Iowa State Univ., Ames, IA (United States)

    2012-01-01

    The purpose of my dissertation is to understand the structural and magnetic properties of the newly discovered FeAs-based superconductors and the interconnection between superconductivity, antiferromagnetism, and structure. X-ray and neutron scattering techniques are powerful tools to directly observe the structure and magnetism in this system. I used both x-ray and neutron scattering techniques on different transition substituted BaFe2As2 compounds in order to investigate the substitution dependence of structural and magnetic transitions and try to understand the connections between them.

  5. Construction of a magnetic bottle spectrometer and its application to pulse duration measurement of X-ray laser using a pump-probe method

    Directory of Open Access Journals (Sweden)

    S. Namba

    2015-11-01

    Full Text Available To characterize the temporal evolution of ultrashort X-ray pulses emitted by laser plasmas using a pump-probe method, a magnetic bottle time-of-flight electron spectrometer is constructed. The design is determined by numerical calculations of a mirror magnetic field and of the electron trajectory in a flight tube. The performance of the spectrometer is characterized by measuring the electron spectra of xenon atoms irradiated with a laser-driven plasma X-ray pulse. In addition, two-color above-threshold ionization (ATI experiment is conducted for measurement of the X-ray laser pulse duration, in which xenon atoms are simultaneously irradiated with an X-ray laser pump and an IR laser probe. The correlation in the intensity of the sideband spectra of the 4d inner-shell photoelectrons and in the time delay of the two laser pulses yields an X-ray pulse width of 5.7 ps, in good agreement with the value obtained using an X-ray streak camera.

  6. Protein dynamics in an intermediate state of myoglobin: optical absorption, resonance Raman spectroscopy, and x-ray structure analysis.

    OpenAIRE

    N. Engler; Ostermann, A; Gassmann, A.; Lamb, D C; Prusakov, V E; J. Schott; Schweitzer-Stenner, R; Parak, F. G.

    2000-01-01

    A metastable state of myoglobin is produced by reduction of metmyoglobin at low temperatures. This is done either by irradiation with x-rays at 80 K or by electron transfer from photoexcited tris(2, 2'-bipyridine)-ruthenium(II) at 20 K. At temperatures above 150 K, the conformational transition toward the equilibrium deoxymyoglobin is observed. X-ray crystallography, Raman spectroscopy, and temperature-dependent optical absorption spectroscopy show that the metastable state has a six-ligated ...

  7. Spontaneous current sheets in magnetic fields with applications to stellar X-rays

    CERN Document Server

    Parker, Eugene N

    1994-01-01

    Expanding upon the ideas first proposed in his seminal book Cosmical Magnetic Fields, Eugene N. Parker here offers the first in-depth treatment of the magnetohydrodynamic theory of spontaneous magnetic discontinuities. In detailing his theory of the spontaneous formation of tangential discontinuities (current sheets) in a magnetic field embedded in highly conducting plasma, Parker shows how it can be used to explain the activity of the external magnetic fields of planets, stars, interstellar gas clouds, and galaxies, as well as the magnetic fields in laboratory plasmas. Provocative and fascinating, Spontaneous Current Sheets in Magnetic Fields presents a bold new theory that will excite interest and discussion throughout the space physics community.

  8. Stopping Narrow-Band X-Ray Pulses in Nuclear Media

    Science.gov (United States)

    Kong, Xiangjin; Pálffy, Adriana

    2016-05-01

    A control mechanism for stopping x-ray pulses in resonant nuclear media is investigated theoretically. We show that narrow-band x-ray pulses can be mapped and stored as nuclear coherence in a thin-film planar x-ray cavity with an embedded 57Fe nuclear layer. The pulse is nearly resonant to the 14.4 keV Mössbauer transition in the 57Fe nuclei. The role of the control field is played here by a hyperfine magnetic field which induces interference effects reminiscent of electromagnetically induced transparency. We show that, by switching off the control magnetic field, a narrow-band x-ray pulse can be completely stored in the cavity for approximately 100 ns. Additional manipulation of the external magnetic field can lead to both group velocity and phase control of the pulse in the x-ray cavity sample.

  9. Energy and symmetry of dd excitations in undoped layered cuprates measured by Cu L{sub 3} resonant inelastic x-ray scattering

    Energy Technology Data Exchange (ETDEWEB)

    Moretti Sala, M; Minola, M [CNISM and Dipartimento di Fisica, Politecnico di Milano, Piazza Leonardo da Vinci 32, I-20133 Milano (Italy); Bisogni, V; Brookes, N B [European Synchrotron Radiation Facility, BoIte Postale 220, F-38043 Grenoble (France); Aruta, C; Luca, G M de; Miletto Granozio, F; Perna, P; Radovic, M; Salluzzo, M [CNR-SPIN and Dipartimento di Scienze Fisiche, Universita di Napoli ' Federico II' , Complesso di Monte S Angelo, Via Cinthia, I-80126 Napoli (Italy); Balestrino, G; Di Castro, D; Medaglia, P G [CNR-SPIN and Dipartimento di Ingegneria Meccanica, Universita di Roma Tor Vergata, Via del Politecnico 1, I-00133 Roma (Italy); Berger, H; Grioni, M; Guarise, M [Ecole Polytechnique Federale de Lausanne (EPFL), Institut de Physique de la Matiere Condensee, CH-1015 Lausanne (Switzerland); Schmitt, T; Zhou, K J [Swiss Light Source, Paul Scherrer Institut, CH-5232 Villigen PSI (Switzerland); Braicovich, L; Ghiringhelli, G, E-mail: marco.moretti@esrf.fr [CNR-SPIN and Dipartimento di Fisica, Politecnico di Milano, piazza Leonardo da Vinci 32, I-20133 Milano (Italy)

    2011-04-15

    We measured the high-resolution Cu L{sub 3} edge resonant inelastic x-ray scattering (RIXS) of undoped cuprates La{sub 2}CuO{sub 4}, Sr{sub 2}CuO{sub 2}Cl{sub 2}, CaCuO{sub 2} and NdBa{sub 2}Cu{sub 3}O{sub 6}. The dominant spectral features were assigned to dd excitations and we extensively studied their polarization and scattering geometry dependence. In a pure ionic picture, we calculated the theoretical cross sections for those excitations and used these to fit the experimental data with excellent agreement. By doing so, we were able to determine the energy and symmetry of Cu-3d states for the four systems with unprecedented accuracy and confidence. The values of the effective parameters could be obtained for the single-ion crystal field model but not for a simple two-dimensional cluster model. The firm experimental assessment of dd excitation energies carries important consequences for the physics of high-T{sub c} superconductors. On the one hand, we found that the minimum energy of orbital excitation is always {>=}1.4 eV, i.e. well above the mid-infrared spectral range, which leaves to magnetic excitations (up to 300 meV) a major role in Cooper pairing in cuprates. On the other hand, it has become possible to study quantitatively the effective influence of dd excitations on the superconducting gap in cuprates.

  10. GROUND-STATE OF FERROMAGNETIC NICKEL AND MAGNETIC CIRCULAR-DICHROISM IN 2P AND 3P CORE X-RAY ABSORPTION SPECTROSCOPIES

    NARCIS (Netherlands)

    JO, T; YOSHIDA, A; SAWATZKY, GA

    The electronic state of ferromagnetic Ni and an interpretation of magnetic circular dichroism (MCD) in Ni 2p --> 3d and 3p --> 3d X-ray absorption (XAS) are discussed from a viewpoint of 3d configuration interaction. Inclusion of the 3d8 configuration and an orbital-magnetic-moment contribution of

  11. Comparison of the magnetic properties of GeMn thin films through Mn L-edge x-ray absorption

    Energy Technology Data Exchange (ETDEWEB)

    Ahlers, S.; Stone, P.R.; Sircar, N.; Arenholz, E.; Dubon, O. D.; Bougeard, D.

    2009-08-04

    X-ray absorption spectroscopy of epitaxial GeMn thin films reveals an experimentally indistinguishable electronic configuration of Mn atoms incorporated in Ge{sub 1?x}Mn{sub x} nanoclusters and in precipitates of the intermetallic compound Mn{sub 5}Ge{sub 3}, respectively. However, the average magnetic response of thin films containing Ge{sub 1?x}Mn{sub x} nanoclusters is lower than the response of films containing Mn{sub 5}Ge{sub 3} precipitates. This reduced magnetic response of Ge{sub 1?x}Mn{sub x} nanoclusters is explained in terms of a fraction of Mn atoms being magnetically inactive due to antiferromagnetic coupling or the presence of structural disorder. A determination of the role of magnetically inactive Mn atoms in the self-assembly of the thermodynamically metastable Ge{sub 1?x}Mn{sub x} nanoclusters seems to be an essential ingredient for an enhanced control of this promising high Curie temperature magnetic semiconductor.

  12. X-ray absorption and resonance raman spectroscopy of human myeloperoxidase at neutral and acid pH.

    Science.gov (United States)</