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Sample records for resolved x-ray laser

  1. Laser plasma x-ray source for ultrafast time-resolved x-ray absorption spectroscopy

    Directory of Open Access Journals (Sweden)

    L. Miaja-Avila

    2015-03-01

    Full Text Available We describe a laser-driven x-ray plasma source designed for ultrafast x-ray absorption spectroscopy. The source is comprised of a 1 kHz, 20 W, femtosecond pulsed infrared laser and a water target. We present the x-ray spectra as a function of laser energy and pulse duration. Additionally, we investigate the plasma temperature and photon flux as we vary the laser energy. We obtain a 75 μm FWHM x-ray spot size, containing ∼106 photons/s, by focusing the produced x-rays with a polycapillary optic. Since the acquisition of x-ray absorption spectra requires the averaging of measurements from >107 laser pulses, we also present data on the source stability, including single pulse measurements of the x-ray yield and the x-ray spectral shape. In single pulse measurements, the x-ray flux has a measured standard deviation of 8%, where the laser pointing is the main cause of variability. Further, we show that the variability in x-ray spectral shape from single pulses is low, thus justifying the combining of x-rays obtained from different laser pulses into a single spectrum. Finally, we show a static x-ray absorption spectrum of a ferrioxalate solution as detected by a microcalorimeter array. Altogether, our results demonstrate that this water-jet based plasma source is a suitable candidate for laboratory-based time-resolved x-ray absorption spectroscopy experiments.

  2. Time-resolved x-ray spectra of laser irradiated high-Z targets

    International Nuclear Information System (INIS)

    Lee, P.H.Y.; Attwood, D.T.; Boyle, M.J.; Campbell, E.M.; Coleman, L.C.; Kornblum, H.N.

    1977-01-01

    Recent results obtained by using the Livermore 15 psec x-ray streak camera to record x-ray emission from laser-irradiated high-z targets in the 1-20 keV range are reported. Nine to eleven K-edge filter channels were used for the measurements. In the lower energy channels, a dynamic range of x-ray emission intensity of better than three orders of magnitude have been recorded. Data will be presented which describe temporally and spectrally resolved x-ray spectra of gold disk targets irradiated by laser pulses from the Argus facility, including the temporal evolution of the superthermal x-ray tail

  3. Time-resolved x-ray line diagnostics of laser-produced plasmas

    International Nuclear Information System (INIS)

    Kauffman, R.L.; Matthews, D.L.; Kilkenny, J.D.; Lee, R.W.

    1982-11-01

    We have examined the underdense plasma conditions of laser irradiated disks using K x-rays from highly ionized ions. A 900 ps laser pulse of 0.532 μm light is used to irradiate various Z disks which have been doped with low concentrations of tracer materials. The tracers, whose Z's range from 13 to 22, are chosen so that their K x-ray spectrum is sensitive to typical underdense plasma temperatures and densities. Spectra are measured using a time-resolved crystal spectrograph recording the time history of the x-ray spectrum. A spatially-resolved, time-integrated crystal spectrograph also monitors the x-ray lines. Large differences in Al spectra are observed when the host plasms is changed from SiO 2 to PbO or In. Spectra will be presented along with preliminary analysis of the data

  4. Time-resolved x-ray line diagnostics of laser-produced plasmas

    International Nuclear Information System (INIS)

    Kauffman, R.L.; Matthews, D.L.; Kilkenny, J.D.; Lee, R.W.

    1982-01-01

    We have examined the underdense plasma conditions of laser irradiated disks using K x-rays from highly ionized ions. A 900 ps laser pulse of 0.532 μm light is used to irradiate various Z disks which have been doped with low concentrations of tracer materials. The tracers whose Z's range from 13 to 22 are chosen so that their K x-ray spectrum is sensitive to typical underdense plasma temperatures and densities. Spectra are measured using a time-resolved crystal spectrograph recording the time history of the x-ray spectrum. A spatially-resolved, time-integrated crystal spectrograph also monitors the x-ray lines. Large differences in Al spectra are observed when the host plasma is changed from SiO 2 to PbO or In. Spectra will be presented along with preliminary analysis of the data

  5. Time-resolved protein nano-crystallography using an X-ray free-electron laser

    International Nuclear Information System (INIS)

    Aquila, Andrew; Hunter, Mark S.; Fromme, Petra; Fromme, Raimund; Grotjohann, Ingo; Doak, R. Bruce; Kirian, Richard A.; Schmidt, Kevin E.; Wang, Xiaoyu; Weierstall, Uwe; Spence, John C.H.; White, Thomas A.; Caleman, Carl; DePonte, Daniel P.; Fleckenstein, Holger; Gumprecht, Lars; Liang, Mengning; Martin, Andrew V.; Schulz, Joachim; Stellato, Francesco; Stern, Stephan; Barty, Anton; Andreasson, Jakob; Davidsson, Jan; Hajdu, Janos; Maia, Filipe R.N.C.; Seibert, M. Marvin; Timneanu, Nicusor; Arnlund, David; Johansson, Linda; Malmerberg, Erik; Neutze, Richard; Bajt, Sasa; Barthelmess, Miriam; Graafsma, Heinz; Hirsemann, Helmut; Wunderer, Cornelia; Barends, Thomas R.M.; Foucar, Lutz; Krasniqi, Faton; Lomb, Lukas; Rolles, Daniel; Schlichting, Ilme; Schmidt, Carlo; Bogan, Michael J.; Hampton, Christina Y.; Sierra, Raymond; Starodub, Dmitri; Bostedt, Christoph; Bozek, John D.; Messerschmidt, Marc; Williams, Garth J.; Bottin, Herve

    2012-01-01

    We demonstrate the use of an X-ray free electron laser synchronized with an optical pump laser to obtain X-ray diffraction snapshots from the photo-activated states of large membrane protein complexes in the form of nano-crystals flowing in a liquid jet. Light-induced changes of Photosystem I-Ferredoxin co-crystals were observed at time delays of 5 to 10 μs after excitation. The result correlates with the microsecond kinetics of electron transfer from Photosystem I to ferredoxin. The undocking process that follows the electron transfer leads to large rearrangements in the crystals that will terminally lead to the disintegration of the crystals. We describe the experimental setup and obtain the first time resolved femtosecond serial X-ray crystallography results from an irreversible photo-chemical reaction at the Linac Coherent Light Source. This technique opens the door to time-resolved structural studies of reaction dynamics in biological systems. (authors)

  6. Time-resolved x-ray laser induced photoelectron spectroscopy of isochoric heated copper

    International Nuclear Information System (INIS)

    Nelson, A.J.; Dunn, J.; Hunter, J.; Widmann, K.

    2005-01-01

    Time-resolved x-ray photoelectron spectroscopy is used to probe the nonsteady-state evolution of the valence band electronic structure of laser heated ultrathin (50 nm) copper. A metastable phase is studied using a 527 nm wavelength 400 fs laser pulse containing 0.1-2.5 mJ laser energy focused in a large 500x700 μm 2 spot to create heated conditions of 0.07-1.8x10 12 W cm -2 intensity. Valence band photoemission spectra are presented showing the changing occupancy of the Cu 3d level with heating are presented. These picosecond x-ray laser induced time-resolved photoemission spectra of laser-heated ultrathin Cu foil show dynamic changes in the electronic structure. The ultrafast nature of this technique lends itself to true single-state measurements of shocked and heated materials

  7. Time-resolved soft x-ray spectra from laser-produced Cu plasma

    International Nuclear Information System (INIS)

    Cone, K.V.; Dunn, J.; Baldis, H.A.; May, M.J.; Purvis, M.A.; Scott, H.A.; Schneider, M.B.

    2012-01-01

    The volumetric heating of a thin copper target has been studied with time resolved x-ray spectroscopy. The copper target was heated from a plasma produced using the Lawrence Livermore National Laboratory's Compact Multipulse Terrawatt (COMET) laser. A variable spaced grating spectrometer coupled to an x-ray streak camera measured soft x-ray emission (800-1550 eV) from the back of the copper target to characterize the bulk heating of the target. Radiation hydrodynamic simulations were modeled in 2-dimensions using the HYDRA code. The target conditions calculated by HYDRA were post-processed with the atomic kinetics code CRETIN to generate synthetic emission spectra. A comparison between the experimental and simulated spectra indicates the presence of specific ionization states of copper and the corresponding electron temperatures and ion densities throughout the laser-heated copper target.

  8. Visualizing a protein quake with time-resolved X-ray scattering at a free-electron laser

    DEFF Research Database (Denmark)

    Arnlund, David; Johansson, Linda C.; Wickstrand, Cecilia

    2014-01-01

    We describe a method to measure ultrafast protein structural changes using time-resolved wide-angle X-ray scattering at an X-ray free-electron laser. We demonstrated this approach using multiphoton excitation of the Blastochloris viridis photosynthetic reaction center, observing an ultrafast glob...

  9. An iterative method for unfolding time-resolved soft x-ray spectra of laser plasmas

    International Nuclear Information System (INIS)

    Tang Yongjian; Shen Kexi; Xu Hepin

    1991-01-01

    Dante-recorded temporal waveforms have been unfolded by using Fast Fourier transformation (FFT) and the inverted convolution theorem of Fourier analysis. The conversion of the signals to time-dependent soft x-ray spectra is accomplished on the IBM-PC/XT-286 microcomputer system with the code DTSP including SAND II reported by W.N.Mcelory et al.. An amplitude-limited iterative and periodic smoothing technique has been developed in the code DTSP. Time-resolved soft x-ray spectra with sixteen time-cell, and time-dependent radiation, [T R (t)], have been obtained for hohlraum targets irradiated with laser beams (λ = 1.06 μm) on LF-12 in 1989

  10. Time-resolved X-ray diffraction with accelerator- and laser-plasma-based X-ray sources

    International Nuclear Information System (INIS)

    Nicoul, Matthieu

    2010-01-01

    Femtosecond X-ray pulses are a powerful tool to investigate atomic motions triggered by femtosecond pump pulses. This thesis is dedicated to the production of such pulses and their use in optical pump - X-ray probe measurement. This thesis describes the laser-plasma-based sources available at the University of Duisburg-Essen. Part of it consists of the description of the design, built-up and characterization of a new ''modular'' X-ray source dedicated to optimize the X-ray flux onto the sample under investigation. The acoustic wave generation in femtosecond optically excited semiconductor (gallium arsenide) and metal (gold) was performed using the sources of the University of Duisburg-Essen. The physical answer of the material was modeled by a simple strain model for the semiconductor, pressure model for the metal, in order to gain information on the interplay of the electronic and thermal pressures rising after excitation. Whereas no reliable information could be obtain in gallium arsenide (principally due to the use of a bulk), the model for gold achieved very good agreement, providing useful information. The relaxation time of the electron to lattice energy was found to be (5.0±0.3) ps, and the ratio of the Grueneisen parameters was found to be γ e / γ i = (0.5±0.1). This thesis also describes the Sub-Picosecond Pulse Source (SPPS) which existed at the (formally) Stanford Linear Accelerator Center, an accelerator-based X-ray source, and two measurements performed with it. The first one is the detailed investigation of the phonon softening of the A 1g mode launch in bismuth upon fluence excitation. Detailed information concerning the new equilibrium position and phonon frequency were obtained over extended laser pump fluences. The second measurement concerned the study of the liquid phase dynamics in a newly formed liquid phase following ultrafast melting in indium antimonide. The formation of the liquid phase and its development for excitations close to the

  11. Time-resolved X-ray diffraction with accelerator- and laser-plasma-based X-ray sources

    Energy Technology Data Exchange (ETDEWEB)

    Nicoul, Matthieu

    2010-09-01

    Femtosecond X-ray pulses are a powerful tool to investigate atomic motions triggered by femtosecond pump pulses. This thesis is dedicated to the production of such pulses and their use in optical pump - X-ray probe measurement. This thesis describes the laser-plasma-based sources available at the University of Duisburg-Essen. Part of it consists of the description of the design, built-up and characterization of a new ''modular'' X-ray source dedicated to optimize the X-ray flux onto the sample under investigation. The acoustic wave generation in femtosecond optically excited semiconductor (gallium arsenide) and metal (gold) was performed using the sources of the University of Duisburg-Essen. The physical answer of the material was modeled by a simple strain model for the semiconductor, pressure model for the metal, in order to gain information on the interplay of the electronic and thermal pressures rising after excitation. Whereas no reliable information could be obtain in gallium arsenide (principally due to the use of a bulk), the model for gold achieved very good agreement, providing useful information. The relaxation time of the electron to lattice energy was found to be (5.0{+-}0.3) ps, and the ratio of the Grueneisen parameters was found to be {gamma}{sub e} / {gamma}{sub i} = (0.5{+-}0.1). This thesis also describes the Sub-Picosecond Pulse Source (SPPS) which existed at the (formally) Stanford Linear Accelerator Center, an accelerator-based X-ray source, and two measurements performed with it. The first one is the detailed investigation of the phonon softening of the A{sub 1g} mode launch in bismuth upon fluence excitation. Detailed information concerning the new equilibrium position and phonon frequency were obtained over extended laser pump fluences. The second measurement concerned the study of the liquid phase dynamics in a newly formed liquid phase following ultrafast melting in indium antimonide. The formation of the liquid phase

  12. Space- and time-resolved diagnostics of soft x-ray emission from laser plasmas

    International Nuclear Information System (INIS)

    Richardson, M.C.; Jaanimagi, P.A.; Chen, H.

    1988-01-01

    The analysis of soft x-ray emission from plasmas created by intense short-wavelength laser radiation can provide much useful information on the density, temperature and ionization distribution of the plasma. Until recently, limitations of sensitivity and the availability of suitable x-ray optical elements have restricted studies of soft x-ray emission from laser plasmas. In this paper, the authors describe novel instrumentation which provides high sensitivity in the soft x-ray spectrum with spatial and temporal resolution in the micron and picosecond ranges respectively. These systems exploit advances made in soft x-ray optic and electro-optic technology. Their application in current studies of laser fusion, x-ray lasers, and high density atomic physics are discussed

  13. Time resolved x-ray pinhole photography of compressed laser fusion targets

    International Nuclear Information System (INIS)

    Attwood, D.T.

    1976-01-01

    Use of the Livermore x-ray streak camera to temporally record x-ray pinhole images of laser compressed targets is described. Use is made of specially fabricated composite x-ray pinholes which are near diffraction limited for 6 A x-rays, but easily aligned with a He--Ne laser of 6328 A wavelength. With a 6 μm x-ray pinhole, the overall system can be aligned to 5 μm accuracy and provides implosion characteristics with space--time resolutions of approximately 6 μm and 15 psec. Acceptable criteria for pinhole alignment, requisite x-ray flux, and filter characteristics are discussed. Implosion characteristics are presented from our present experiments with 68 μm diameter glass microshell targets and 0.45 terawatt, 70 psec Nd laser pulses. Final implosion velocities in excess of 3 x 10 7 cm/sec are evident

  14. Diagnosis of laser ablated carbon particles measured by time-resolved X-ray absorption spectroscopy

    International Nuclear Information System (INIS)

    Miyashita, Atsumi; Yoda, Osamu; Ohyanagi, T.; Murakami, K.

    1995-01-01

    The time and space resolved properties of laser ablated carbon particles were measured by X-ray absorption spectroscopy using LPX as an X-ray source. The energy density of the irradiation laser on the sample was in the range of 0.5-20J/cm 2 and the time delay was varied between 0 and 120ns. The absorption spectra exhibited several peaks originated from level to level transitions and an intense broad absorption in the energy range of C-K edge. At a delay time of 120ns, the absorption peak from 1s→2p transition of neutral carbon atom (C 0 ), C - , C + and C 2+ ions were observed. The absorption peak from C 0 was stronger as the probing position was closer to the sample surface and decreased rapidly with distance from the sample surface. The absorption peak C 2+ ion was observed only at comparatively distant positions from surface. The maximum speeds of highly charged ions were faster than that of neutral atoms and negative charged ions. The neutral atom and lower charged ions were emitted from the sample even after laser irradiation. The spatial distributions of the laser ablated carbon particles in the localized helium gas environment were measured. In the helium gas environment, the ablation plume was depressed by the helium cloud generated on the top of ablation plume. (author)

  15. Spatially and temporally resolved x-ray emission from imploding laser fusion targets

    International Nuclear Information System (INIS)

    Attwood, D.T.; Coleman, L.W.; Boyle, M.J.; Phillion, D.W.; Swain, J.E.; Manes, K.R.; Larsen, J.T.

    1976-09-01

    The Livermore 15 psec x-ray streak camera has been used in conjunction with 6 μm diameter pinholes to record well resolved implosion histories of DT filled laser fusion targets. The space-time compression data provide clearly identified implosion velocities, typically 3 x 10 7 cm/sec for two-sided clamshell irradiation of a 70 μm/sup D/, .5 μm wall DT filled glass microshell. Single-sided irradiation results show hydrodynamic convergence at the target center, followed by an asymmetric but two-sided target disassembly. These experiments were performed at the two arm Janus Laser facility, which typically delivered a total of 0.4 TW in a 70 psec pulse for these experiments

  16. X-ray lasers

    CERN Document Server

    Elton, Raymond C

    2012-01-01

    The first in its field, this book is both an introduction to x-ray lasers and a how-to guide for specialists. It provides new entrants and others interested in the field with a comprehensive overview and describes useful examples of analysis and experiments as background and guidance for researchers undertaking new laser designs. In one succinct volume, X-Ray Lasers collects the knowledge and experience gained in two decades of x-ray laser development and conveys the exciting challenges and possibilities still to come._Add on for longer version of blurb_M>The reader is first introduced

  17. Time resolved measurement of laser-ablated particles by LAPXAS (Laser Plasma Soft X-ray Absorption Spectroscopy)

    International Nuclear Information System (INIS)

    Miyashita, Atsumi; Yoda, Osamu; Murakami, Kouichi

    1999-01-01

    The time- and spatially-resolved properties of laser ablated carbon, boron and silicon particles were measured by LAPXAS (Laser Plasma Soft X-ray Absorption Spectroscopy). The maximum speed of positively charged ions is higher than those of neutral atoms and negatively charged ions. The spatial distributions of the laser-ablated particles in the localized rare gas environment were measured. In helium gas environment, by the helium cloud generated on the top of ablation plume depressed the ablation plume. There is no formation of silicon clusters till 15 μs after laser ablation in the argon gas environment. (author)

  18. Introducing a standard method for experimental determination of the solvent response in laser pump, x-ray probe time-resolved wide-angle x-ray scattering experiments on systems in solution

    DEFF Research Database (Denmark)

    Kjær, Kasper Skov; Brandt van Driel, Tim; Kehres, Jan

    2013-01-01

    In time-resolved laser pump, X-ray probe wide-angle X-ray scattering experiments on systems in solution the structural response of the system is accompanied by a solvent response. The solvent response is caused by reorganization of the bulk solvent following the laser pump event, and in order...... response-the solvent term-experimentally when applying laser pump, X-ray probe time-resolved wide-angle X-ray scattering. The solvent term describes difference scattering arising from the structural response of the solvent to changes in the hydrodynamic parameters: pressure, temperature and density. We...... is demonstrated to exhibit first order behaviour with respect to the amount of energy deposited in the solution. We introduce a standardized method for recording solvent responses in laser pump, X-ray probe time-resolved X-ray wide-angle scattering experiments by using dye mediated solvent heating. Furthermore...

  19. Spatially resolved x-ray laser spectra and demonstration of gain in nickel-like systems

    Energy Technology Data Exchange (ETDEWEB)

    Whelan, D.A.; Keane, C.J.; MacGowan, B.J.; Matthews, D.L.; Trebes, J.E.; Eckart, M.J.

    1987-09-25

    A recent series of experiments have provided spatially resolved near field images of several candidate x-ray lasing transition in neon-like, nickel-like, and hydrogen-like ions from laser-produced plasmas. From these time-gated, spatially, and spectrally resolved measurements the source size for the J = 0 - 1 and the J = 2 - 1 transitions in Ne-like selenium have been determined. Source regions as small as 50 ..mu..m have been observed on transitions with gain-length products >9. In addition, we have obtained the first experimental evidence for the amplification of spontaneous emission in the nickel-like ions of europium and ytterbium. Gains of order 1 cm/sup -1/ and gain-length products of up to 3.8 are observed on the J = 0 - 1, 4d-4p transitions in Eu + 35 at 65.26 and 71.00 A. Analogous transitions in Yb = +42 have been identified and some evidence for ASE has been observed. 7 refs., 11 figs.

  20. Spatially resolved X-ray laser spectra and demonstration of gain in nickel-like systems

    International Nuclear Information System (INIS)

    Whelan, D.A.; Keane, C.J.; MacGowan, B.J.; Matthews, D.L.; Trebes, J.E.; Eckart, M.J.

    1987-01-01

    A recent series of experiments have provided spatially resolved near field images of several candidate x-ray lasing transition in neon-like, nickel-like, and hydrogen-like ions from laser-produced plasmas. From these time-gated, spatially, and spectrally resolved measurements the source size for the J=0-1 and the J=2-1 transitions in Ne-like selenium have been determined. Source regions as small as 50 μm have been observed on transitions with gain-length products >9. In addition, the authors have obtained the first experimental evidence for the amplification of spontaneous emission in the nickel-like ions of europium and ytterbium. Gains of order 1 cm/sup -1/ and gain-length products of up to 3.8 are observed on the J=0-1,4d-4p transitions in Eu/sup +35/ at 65.83 and 71.00A. Analogous transitions in Yb/sup +42/ have been identified and some evidence for ASE has been observed

  1. Time-resolved soft-x-ray studies of energy transport in layered and planar laser-driven targets

    International Nuclear Information System (INIS)

    Stradling, G.L.

    1982-01-01

    New low-energy x-ray diagnostic techniques are used to explore energy-transport processes in laser heated plasmas. Streak cameras are used to provide 15-psec time-resolution measurements of subkeV x-ray emission. A very thin (50 μg/cm 2 ) carbon substrate provides a low-energy x-ray transparent window to the transmission photocathode of this soft x-ray streak camera. Active differential vacuum pumping of the instrument is required. The use of high-sensitivity, low secondary-electron energy-spread CsI photocathodes in x-ray streak cameras is also described. Significant increases in sensitivity with only a small and intermittant decrease in dynamic range were observed. These coherent, complementary advances in subkeV, time-resolved x-ray diagnostic capability are applied to energy-transport investigations of 1.06-μm laser plasmas. Both solid disk targets of a variety of Z's as well as Be-on-Al layered-disk targets were irradiated with 700-psec laser pulses of selected intensity between 3 x 10 14 W/cm 2 and 1 x 10 15 W/cm 2

  2. Time-resolved suprathermal x-rays

    International Nuclear Information System (INIS)

    Lee, P.H.Y.; Rosen, M.D.

    1978-01-01

    Temporally resolved x-ray spectra in the range of 1 to 20 keV have been obtained from gold disk targets irradiated by 1.06 μm laser pulses from the Argus facility. The x-ray streak camera used for the measurement has been calibrated for streak speed and dynamic range by using an air-gap Fabry-Perot etalon, and the instrument response has been calibrated using a multi-range monoenergetic x-ray source. The experimental results indicate that we are able to observe the ''hot'' x-ray temperature evolve in time and that the experimentally observed values can be qualitatively predicted by LASNEX code computations when the inhibited transport model is used

  3. Laser wakefield generated X-ray probe for femtosecond time-resolved measurements of ionization states of warm dense aluminum

    Energy Technology Data Exchange (ETDEWEB)

    Mo, M. Z.; Chen, Z.; Tsui, Y. Y.; Fedosejevs, R. [Department of Electrical and Computer Engineering, University of Alberta, Edmonton, Alberta T6G 2V4 (Canada); Fourmaux, S.; Saraf, A.; Otani, K.; Kieffer, J. C. [INRS-EMT, Université du Québec, 1650 Lionel Boulet, Varennes, Québec J3X 1S2 (Canada); Ng, A. [Department of Physics and Astronomy, University of British Columbia, British Columbia V6T 1Z1 (Canada)

    2013-12-15

    We have developed a laser wakefield generated X-ray probe to directly measure the temporal evolution of the ionization states in warm dense aluminum by means of absorption spectroscopy. As a promising alternative to the free electron excited X-ray sources, Betatron X-ray radiation, with femtosecond pulse duration, provides a new technique to diagnose femtosecond to picosecond transitions in the atomic structure. The X-ray probe system consists of an adjustable Kirkpatrick-Baez (KB) microscope for focusing the Betatron emission to a small probe spot on the sample being measured, and a flat Potassium Acid Phthalate Bragg crystal spectrometer to measure the transmitted X-ray spectrum in the region of the aluminum K-edge absorption lines. An X-ray focal spot size of around 50 μm was achieved after reflection from the platinum-coated 10-cm-long KB microscope mirrors. Shot to shot positioning stability of the Betatron radiation was measured resulting in an rms shot to shot variation in spatial pointing on the sample of 16 μm. The entire probe setup had a spectral resolution of ∼1.5 eV, a detection bandwidth of ∼24 eV, and an overall photon throughput efficiency of the order of 10{sup −5}. Approximately 10 photons were detected by the X-ray CCD per laser shot within the spectrally resolved detection band. Thus, it is expected that hundreds of shots will be required per absorption spectrum to clearly observe the K-shell absorption features expected from the ionization states of the warm dense aluminum.

  4. Soft x-ray lasers

    International Nuclear Information System (INIS)

    Matthews, D.L.; Rosen, M.D.

    1988-01-01

    One of the elusive dreams of laser physicists has been the development of an x-ray laser. After 25 years of waiting, the x-ray laser has at last entered the scientific scene, although those now in operation are still laboratory prototypes. They produce soft x rays down to about five nanometers. X-ray lasers retain the usual characteristics of their optical counterparts: a very tight beam, spatial and temporal coherence, and extreme brightness. Present x-ray lasers are nearly 100 times brighter that the next most powerful x-ray source in the world: the electron synchrotron. Although Lawrence Livermore National Laboratory (LLNL) is widely known for its hard-x-ray laser program which has potential applications in the Strategic Defense Initiative, the soft x-ray lasers have no direct military applications. These lasers, and the scientific tools that result from their development, may one day have a place in the design and diagnosis of both laser fusion and hard x-ray lasers. The soft x-ray lasers now in operation at the LLNL have shown great promise but are still in the primitive state. Once x-ray lasers become reliable, efficient, and economical, they will have several important applications. Chief among them might be the creation of holograms of microscopic biological structures too small to be investigated with visible light. 5 figs

  5. Time-resolved x-ray diagnostics

    International Nuclear Information System (INIS)

    Lyons, P.B.

    1981-01-01

    Techniques for time-resolved x-ray diagnostics will be reviewed with emphasis on systems utilizing x-ray diodes or scintillators. System design concerns for high-bandwidth (> 1 GHz) diagnostics will be emphasized. The limitations of a coaxial cable system and a technique for equalizing to improve bandwidth of such a system will be reviewed. Characteristics of new multi-GHz amplifiers will be presented. An example of a complete operational system on the Los Alamos Helios laser will be presented which has a bandwidth near 3 GHz over 38 m of coax. The system includes the cable, an amplifier, an oscilloscope, and a digital camera readout

  6. Strategies for Time-resolved X-ray Diffraction of Phase Transitions with Laser Compression

    Science.gov (United States)

    Benedetti, Laura Robin; Eggert, J. H.; Bradley, D. K.; Bell, P. M.; Kilkenny, J. D.; Palmer, N.; Petre, R. B.; Rygg, J. R.; Sorce, C.; Collins, G. W.; Boehly, T. R.

    2017-10-01

    As part of a program to document kinetics of phase transitions under laser-driven dynamic compression, we are designing a platform to make multiple x-ray diffraction measurements during a single laser experiment. Our plans include experimental development at Omega-EP and eventual implementation at NIF. We will present our strategy for designing a robust platform that can effectively document a wide variety of phase transformations by utilizing both streaked and multiple-frame imaging detectors. Preliminary designs utilize a novel CMOS detector designed by Sandia National Lab. Our initial experiments include scoping studies that will focus on photometrics and shielding requirements in the high EMP environment close to the target. This work was performed under the auspices of the U.S. Department of Energy by Lawrence Livermore National Laboratory under Contract DE-AC52-07NA27344. Lawrence Livermore National Security, LLC, LLNL-ABS-734470.

  7. X-Ray Lasers 2016

    CERN Document Server

    Bulanov, Sergei; Daido, Hiroyuki; Kato, Yoshiaki

    2018-01-01

    These proceedings comprise a selection of invited and contributed papers presented at the 15th International Conference on X-Ray Lasers (ICXRL 2016), held at the Nara Kasugano International Forum, Japan, from May 22 to 27, 2016. This conference was part of an ongoing series dedicated to recent developments in the science and technology of x-ray lasers and other coherent x-ray sources with additional focus on supporting technologies, instrumentation and applications.   The book showcases recent advances in the generation of intense, coherent x-rays, the development of practical devices and their applications across a wide variety of fields. It also discusses emerging topics such as plasma-based x-ray lasers, 4th generation accelerator-based sources and higher harmonic generations, as well as other x-ray generation schemes.

  8. Broadband time-resolved elliptical crystal spectrometer for X-ray spectroscopic measurements in laser-produced plasmas

    International Nuclear Information System (INIS)

    Wang Rui-Rong; Jia Guo; Fang Zhi-Heng; Wang Wei; Meng Xiang-Fu; Xie Zhi-Yong; Zhang Fan

    2014-01-01

    The X-ray spectrometer used in high-energy-density plasma experiments generally requires both broad X-ray energy coverage and high temporal, spatial, and spectral resolutions for overcoming the difficulties imposed by the X-ray background, debris, and mechanical shocks. By using an elliptical crystal together with a streak camera, we resolve this issue at the SG-II laser facility. The carefully designed elliptical crystal has a broad spectral coverage with high resolution, strong rejection of the diffuse and/or fluorescent background radiation, and negligible source broadening for extended sources. The spectra that are Bragg reflected (23° < θ < 38°) from the crystal are focused onto a streak camera slit 18 mm long and about 80 μm wide, to obtain a time-resolved spectrum. With experimental measurements, we demonstrate that the quartz(1011) elliptical analyzer at the SG-II laser facility has a single-shot spectral range of (4.64–6.45) keV, a typical spectral resolution of E/ΔE = 560, and an enhanced focusing power in the spectral dimension. For titanium (Ti) data, the lines of interest show a distribution as a function of time and the temporal variations of the He-α and Li-like Ti satellite lines and their spatial profiles show intensity peak red shifts. The spectrometer sensitivity is illustrated with a temporal resolution of better than 25 ps, which satisfies the near-term requirements of high-energy-density physics experiments. (atomic and molecular physics)

  9. Time-resolved x-ray spectra from laser-generated high-density plasmas

    Science.gov (United States)

    Andiel, U.; Eidmann, Klaus; Witte, Klaus-Juergen

    2001-04-01

    We focused frequency doubled ultra short laser pulses on solid C, F, Na and Al targets, K-shell emission was systematically investigated by time resolved spectroscopy using a sub-ps streak camera. A large number of laser shots can be accumulated when triggering the camera with an Auston switch system at very high temporal precision. The system provides an outstanding time resolution of 1.7ps accumulating thousands of laser shots. The time duration of the He-(alpha) K-shell resonance lines was observed in the range of (2-4)ps and shows a decrease with the atomic number. The experimental results are well reproduced by hydro code simulations post processed with an atomic kinetics code.

  10. Picosecond time-resolved laser pump/X-ray probe experiments using a gated single-photon-counting area detector

    DEFF Research Database (Denmark)

    Ejdrup, T.; Lemke, H.T.; Haldrup, Martin Kristoffer

    2009-01-01

    The recent developments in X-ray detectors have opened new possibilities in the area of time-resolved pump/probe X-ray experiments; this article presents the novel use of a PILATUS detector to achieve X-ray pulse duration limited time-resolution at the Advanced Photon Source (APS), USA...... limited time-resolution of 60 ps using the gated PILATUS detector. This is the first demonstration of X-ray pulse duration limited data recorded using an area detector without the use of a mechanical chopper array at the beamline........ The capability of the gated PILATUS detector to selectively detect the signal from a given X-ray pulse in 24 bunch mode at the APS storage ring is demonstrated. A test experiment performed on polycrystalline organic thin films of [alpha]-perylene illustrates the possibility of reaching an X-ray pulse duration...

  11. Time-resolved X-ray absorption spectroscopy for laser-ablated silicon particles in xenon gas

    International Nuclear Information System (INIS)

    Makimura, Tetsuya; Sakuramoto, Tamaki; Murakami, Kouichi

    1996-01-01

    We developed a laboratory-scale in situ apparatus for soft X-ray absorption spectroscopy with a time resolution of 10 ns and a space resolution of 100 μm. Utilizing this spectrometer, we have investigated the dynamics of silicon atoms formed by laser ablation in xenon gas. It was found that 4d-electrons in the xenon atoms are excited through collision with electrons in the laser-generated silicon plasma. (author)

  12. Theory of time-resolved inelastic x-ray diffraction

    DEFF Research Database (Denmark)

    Lorenz, Ulf; Møller, Klaus Braagaard; Henriksen, Niels Engholm

    2010-01-01

    Starting from a general theory of time-resolved x-ray scattering, we derive a convenient expression for the diffraction signal based on a careful analysis of the relevant inelastic scattering processes. We demonstrate that the resulting inelastic limit applies to a wider variety of experimental...... conditions than similar, previously derived formulas, and it directly allows the application of selection rules when interpreting diffraction signals. Furthermore, we present a simple extension to systems simultaneously illuminated by x rays and a laser beam....

  13. Femtosecond X-ray Absorption Spectroscopy at a Hard X-ray Free Electron Laser

    DEFF Research Database (Denmark)

    Lemke, Henrik T.; Bressler, Christian; Chen, Lin X.

    2013-01-01

    X-ray free electron lasers (XFELs) deliver short (current (SASE based) XFELs, they can be used for measuring high......-quality X-ray absorption data and we report femtosecond time-resolved X-ray absorption near-edge spectroscopy (XANES) measurements of a spin-crossover system, iron(II) tris(2,2'-bipyridine) in water. The data indicate that the low-spin to high-spin transition can be modeled by single-exponential kinetics...

  14. Absolutely calibrated, time-resolved measurements of soft x rays using transmission grating spectrometers at the Nike Laser Facility

    International Nuclear Information System (INIS)

    Weaver, J.L.; Feldman, U.; Seely, J.F.; Holland, G.; Serlin, V.; Klapisch, M.; Columbant, D.; Mostovych, A.

    2001-01-01

    Accurate simulation of pellet implosions for direct drive inertial confinement fusion requires benchmarking the codes with experimental data. The Naval Research Laboratory (NRL) has begun to measure the absolute intensity of radiation from laser irradiated targets to provide critical information for the radiatively preheated pellet designs developed by the Nike laser group. Two main diagnostics for this effort are two spectrometers incorporating three detection systems. While both spectrometers use 2500 lines/mm transmission gratings, one instrument is coupled to a soft x-ray streak camera and the other is coupled to both an absolutely calibrated Si photodiode array and a charge coupled device (CCD) camera. Absolute calibration of spectrometer components has been undertaken at the National Synchrotron Light Source at Brookhaven National Laboratories. Currently, the system has been used to measure the spatially integrated soft x-ray flux as a function of target material, laser power, and laser spot size. A comparison between measured and calculated flux for Au and CH targets shows reasonable agreement to one-dimensional modeling for two laser power densities

  15. Small scale soft x-ray lasers

    International Nuclear Information System (INIS)

    Skinner, C.H.; DiCicco, D.S.; Kim, D.; Voorhees, D.; Suckewer, S.

    1990-01-01

    The widespread application of soft x-ray laser technology is contingent on the development of small scale soft x-ray lasers that do not require large laser facilities. Progress in the development of soft x-ray lasers pumped by a Nd laser of energy 6-12J is reported below. Application of an existing soft x-ray laser to x-ray microscopy has begun. A soft x-ray laser of output energy 1-3 mJ at 18,2 nm has been used to record high resolution images of biological specimens. The contact images were recorded on photoresist which was later viewed in a scanning electron microscope. The authors present a composite optical x-ray laser microscope design

  16. Bent crystal spectrometer for both frequency and wavenumber resolved x-ray scattering at a seeded free-electron laser.

    Science.gov (United States)

    Zastrau, Ulf; Fletcher, Luke B; Förster, Eckhart; Galtier, Eric Ch; Gamboa, Eliseo; Glenzer, Siegfried H; Heimann, Philipp; Marschner, Heike; Nagler, Bob; Schropp, Andreas; Wehrhan, Ortrud; Lee, Hae Ja

    2014-09-01

    We present a cylindrically curved GaAs x-ray spectrometer with energy resolution ΔE/E = 1.1 × 10(-4) and wave-number resolution of Δk/k = 3 × 10(-3), allowing plasmon scattering at the resolution limits of the Linac Coherent Light Source (LCLS) x-ray free-electron laser. It spans scattering wavenumbers of 3.6 to 5.2/Å in 100 separate bins, with only 0.34% wavenumber blurring. The dispersion of 0.418 eV/13.5 μm agrees with predictions within 1.3%. The reflection homogeneity over the entire wavenumber range was measured and used to normalize the amplitude of scattering spectra. The proposed spectrometer is superior to a mosaic highly annealed pyrolytic graphite spectrometer when the energy resolution needs to be comparable to the LCLS seeded bandwidth of 1 eV and a significant range of wavenumbers must be covered in one exposure.

  17. Higher coherent x-ray laser

    International Nuclear Information System (INIS)

    Hasegawa, Noboru; Nagashima, Keisuke; Kawachi, Tetsuya

    2001-01-01

    X-ray lasers generated by an ultra short pulse laser have advantages such as monochromatic, short pulse duration, small beam divergence, high intensity, and coherence. Spatial coherence is most important for applications, we have investigated the transient collisional excitation (TCE) scheme x-ray laser lasing from Ne-like titanium (31.6 nm), Ne-like silver (13.9 nm) and tin (11.9 nm). However, the spatial coherence was not so good with this scheme. We have been studying to improve the spatial coherence of the x-ray laser and have proposed to use coherent seed light tuned to the x-ray laser wavelength generated from higher harmonics generation (HHG), which is introduced to the x-ray laser medium (Ne-like titanium, Ni-like silver plasmas). We present about the theoretical study of the coupling efficiency HHG light with x-ray laser medium. (author)

  18. Time-resolved X-ray diffraction studies of laser-induced acoustic wave propagation in bilayer metallic thin crystals

    Energy Technology Data Exchange (ETDEWEB)

    Er, Ali Oguz [Department of Physics and Astronomy, Western Kentucky University, Bowling Green, Kentucky 42101 (United States); Tang, Jau, E-mail: jautang@gate.sinica.edu.tw, E-mail: prentzepis@ece.tamu.edu [Research Center for Applied Sciences Academia Sinica, Taipei, Taiwan (China); Chen, Jie [Key Laboratory for Laser Plasmas (Ministry of Education) and Department of Physics and Astronomy, Shanghai Jiao Tong University, Shanghai 200240 (China); Rentzepis, Peter M., E-mail: jautang@gate.sinica.edu.tw, E-mail: prentzepis@ece.tamu.edu [Department of Electrical and Computer Engineering, Texas A and M University, College Station, Texas 77843 (United States)

    2014-09-07

    Phonon propagation across the interface of a Cu/Ag(111) bilayer and transient lattice disorder, induced by a femtosecond 267 nm pulse, in Ag(111) crystal have been measured by means of time resolved X-ray diffraction. A “blast” force due to thermal stress induced by suddenly heated electrons is formed within two picoseconds after excitation and its “blast wave” propagation through the interface and Ag (111) crystal was monitored by the shift and broadening of the rocking curve, I vs. ω, as a function of time after excitation. Lattice disorder, contraction and expansion as well as thermal strain formation and wave propagation have also been measured. The experimental data and mechanism proposed are supported by theoretical simulations.

  19. Applications of soft x-ray lasers

    International Nuclear Information System (INIS)

    Skinner, C.H.

    1993-01-01

    The high brightness and short pulse duration of soft x-ray lasers provide unique advantages for novel applications. Imaging of biological specimens using x-ray lasers has been demonstrated by several groups. Other applications to fields such as chemistry, material science, plasma diagnostics, and lithography are beginning to emerge. We review the current status of soft x-ray lasers from the perspective of applications, and present an overview of the applications currently being developed

  20. The Livermore X-ray Laser Program

    International Nuclear Information System (INIS)

    Matthews, D.L.

    1992-01-01

    I will report on the status of x-ray laser development and its applications at Livermore. I will review some of our recent results and comment on where our future research is headed including plans for developing a compact x-ray laser users facility. Finally, I will briefly summarize the results of an X-ray Laser Applications Workshop that was held in San Francisco in January 1992

  1. Time-resolved electron beam phase space tomography at a soft x-ray free-electron laser

    Directory of Open Access Journals (Sweden)

    Michael Röhrs

    2009-05-01

    Full Text Available High-gain free-electron lasers (FELs in the ultraviolet and x-ray regime put stringent demands on the peak current, transverse emittance, and energy spread of the driving electron beam. At the soft x-ray FEL FLASH, a transverse deflecting microwave structure (TDS has been installed to determine these parameters for the longitudinally compressed bunches, which are characterized by a narrow leading peak of high charge density and a long tail. The rapidly varying electromagnetic field in the TDS deflects the electrons vertically and transforms the time profile into a streak on an observation screen. The bunch current profile was measured single shot with an unprecedented resolution of 27 fs under FEL operating conditions. A precise single-shot measurement of the energy distribution along a bunch was accomplished by using the TDS in combination with an energy spectrometer. Variation of quadrupole strengths allowed for a determination of the horizontal emittance as a function of the longitudinal position within a bunch, the so-called slice emittance. In the bunch tail, a normalized slice emittance of about 2  μm was found, in agreement with expectations. In the leading spike, however, surprisingly large emittance values were observed, in apparent contradiction with the low emittance deduced from the measured FEL gain. By applying three-dimensional phase space tomography, we were able to show that the bunch head contains a central core of low emittance and high local current density, which is presumably the lasing part of the bunch.

  2. Properties of laser-produced GaAs plasmas measured from highly resolved X-ray line shapes and ratios

    Science.gov (United States)

    Seely, J. F.; Fein, J.; Manuel, M.; Keiter, P.; Drake, P.; Kuranz, C.; Belancourt, Patrick; Ralchenko, Yu.; Hudson, L.; Feldman, U.

    2018-03-01

    The properties of hot, dense plasmas generated by the irradiation of GaAs targets by the Titan laser at Lawrence Livermore National Laboratory were determined by the analysis of high resolution K shell spectra in the 9 keV to 11 keV range. The laser parameters, such as relatively long pulse duration and large focal spot, were chosen to produce a steady-state plasma with minimal edge gradients, and the time-integrated spectra were compared to non-LTE steady state spectrum simulations using the FLYCHK and NOMAD codes. The bulk plasma streaming velocity was measured from the energy shifts of the Ga He-like transitions and Li-like dielectronic satellites. The electron density and the electron energy distribution, both the thermal and the hot non-thermal components, were determined from the spectral line ratios. After accounting for the spectral line broadening contributions, the plasma turbulent motion was measured from the residual line widths. The ionization balance was determined from the ratios of the He-like through F-like spectral features. The detailed comparison of the experimental Ga spectrum and the spectrum simulated by the FLYCHK code indicates two significant discrepancies, the transition energy of a Li-like dielectronic satellite (designated t) and the calculated intensity of a He-like line (x), that should lead to improvements in the kinetics codes used to simulate the X-ray spectra from highly-charged ions.

  3. Atom-resolving x-ray holography

    International Nuclear Information System (INIS)

    Adams, B.; Hiort, T.; Materlik, G.; Nishino, Y.; Novikov, D. V.

    2000-01-01

    The current state of atomic resolution x-ray holography is discussed on the basis of theory and experimental results. X-ray holography is theoretically described in quantum theory. Presently-used experimental implementations are shown together with the data analysis used. Reconstructions of experimental and simulated holograms are compared for a Cu 3 Au crystal structure. Rigorous experimental realizations of pure direct and reciprocal x-ray holography methods are demonstrated, and future developments and applications of the method are suggested

  4. An x-ray technique for precision laser beam synchronization

    International Nuclear Information System (INIS)

    Landen, O.L.; Lerche, R.A.; Hay, R.G.; Hammel, B.A.; Kalantar, D.; Cable, M.D.

    1994-01-01

    A new x-ray technique for recording the relative arrival times of multiple laser beams at a common target with better than ± 10 ps accuracy has been implemented at the Nova laser facility. 100 ps, 3ω Nova beam are focused to separate locations on a gold ribbon target viewed from the side. The measurement consists of using well characterized re-entrant x-ray streak cameras for 1-dimensional streaked imaging of the > 3 keV x-rays emanating from these isolated laser plasmas. After making the necessary correction for the differential laser, x-ray and electron transit times involved, timing offsets as low as ± 7 ps are resolved, and on subsequent shots, corrected for, verified and independently checked. This level of synchronization proved critical in meeting the power balance requirements for indirectly-driven pulse-shaped Nova implosions

  5. Second generation X-ray lasers

    Czech Academy of Sciences Publication Activity Database

    Fajardo, M.; Zeitoun, P.; Faivre, G.; Sebban, S.; Mocek, Tomáš; Hallou, A.; Aubert, D.; Balcou, P.; Burgy, F.; Douillet, D.; Mercere, P.; Morlens, A.S.; Rousseau, J. P.; Valentin, C.; Kazamias, S.; de Lachéze-Murel, G.; Lefrou, T.; Merdji, H.; Le Pape, S.; Ravet, M.F.; Delmotte, F.; Gautier, J.

    2006-01-01

    Roč. 99, 1-3 (2006), s. 142-152 ISSN 0022-4073 Grant - others:NEST-ADVENTURE FP6 EC(XE) project 012841 (TUIXS) Institutional research plan: CEZ:AV0Z10100523 Keywords : X-ray laser * amplification * high harmonic generation * optical field ionization Subject RIV: BH - Optics, Masers, Lasers Impact factor: 1.599, year: 2006

  6. On X-ray laser

    International Nuclear Information System (INIS)

    Durrani, I.R.; Bhatti, Z.R.

    2000-01-01

    Although considerable efforts have been invested in the area of short wavelength lasers at the conceptual and theoretical level for approaching thirty years now it is only with in last two decades that significant progress has been made. The philosophy behind the preparation of this paper has been to indicate to the nonspecialist the fundamental requirements and associated difficulties of achieving laser action. Although we can look to inner shell transitions in neutral or weakly ionized action in this instance the discussion is restricted to the latter possibility. This is mainly because of successful experiments demonstrating amplification using laser produced plasma as a source of lasant ion species. (author)

  7. Saturated output tabletop x-ray lasers

    International Nuclear Information System (INIS)

    Dunn, J.; Osterheld, A.L.; Nilsen, J.; Hunter, J.R.; Li, Y.; Faenov, A.Ya.; Pikuz, T.A.; Shlyaptsev, N.

    2000-01-01

    The high efficiency method of transient collisional excitation has been successfully demonstrated for Ne-like and Ni-like ion x-ray laser schemes with small 5-10 J laser facilities. Our recent studies using the tabletop COMET (Compact Multipulse Terawatt) laser system at the Lawrence Livermore National Laboratory (LLNL) have produced several x-ray lasers operating in the saturation regime. Output energy of 10-15 (micro)J corresponding to a gL product of 18 has been achieved on the Ni-like Pd 4d → 4p transition at 147 (angstrom) with a total energy of 5-7 J in a 600 ps pulse followed by a 1.2 ps pulse. Analysis of the laser beam angular profile indicates that refraction plays an important role in the amplification and propagation process in the plasma column. We report further improvement in the extraction efficiency by varying a number of laser driver parameters. In particular, the duration of the second short pulse producing the inversion has an observed effect on the x-ray laser output

  8. Saturated output tabletop X-ray lasers

    Energy Technology Data Exchange (ETDEWEB)

    Dunn, J.; Osterheld, A.L.; Nilsen, J.; Hunter, J.R. [Lawrence Livermore National Lab., CA (United States); Yuelin Li [Lawrence Livermore National Lab., CA (United States); ILSA, Lawrence Livermore National Lab., Livermore, CA (United States); Faenov, A.Ya.; Pikuz, T.A. [Lawrence Livermore National Lab., CA (United States); MISDC of VNIIFTRI, Mendeleevo (Russian Federation); Shlyaptsev, V.N. [Lawrence Livermore National Lab., CA (United States); DAS, Univ. of California Davis-Livermore, Livermore, CA (United States)

    2001-07-01

    The high efficiency method of transient collisional excitation has been successfully demonstrated for Ne-like and Ni-like ion X-ray laser schemes with small 5-10 J laser facilities. Our recent studies using the tabletop COMET (compact multipulse terawatt) laser system at the Lawrence livermore national laboratory (LLNL) have produced several X-ray lasers operating in the saturation regime. Output energy of 10-15 {mu}J corresponding to a gL product of 18 has been achieved on the Ni-like Pd 4d{yields}4p transition at 147 A with a total energy of 5-7 J in a 600 ps pulse followed by a 1.2 ps pulse. Analysis of the laser beam angular profile indicates that refraction plays an important role in the amplification and propagation process in the plasma column. We report further improvement in the extraction efficiency by varying a number of laser driver parameters. In particular, the duration of the second short pulse producing the inversion has an observed effect on the X-ray laser output. (orig.)

  9. An x-ray detector for time-resolved studies

    International Nuclear Information System (INIS)

    Rodricks, B.; Brizard, C.; Clarke, R.; Lowe, W.

    1992-01-01

    The development of ultrahigh-brightness x-ray sources makes time-resolved x-ray studies more and more feasible. Improvements in x-ray optics components are also critical for obtaining the appropriate beam for a particular type of experiment. Moreover, fast parallel detectors will be essential in order to exploit the combination of high intensity x-ray sources and novel optics for time-resolved experiments. A CCD detector with a time resolution of microseconds has been developed at the Advanced Photon Source (APS). This detector is fully programmable using CAMAC electronics and a Micro Vax computer. The techniques of time-resolved x-ray studies, which include scattering, microradiography, microtomography, stroboscopy, etc., can be applied to a range of phenomena (including rapid thermal annealing, surface ordering, crystallization, and the kinetics of phase transition) in order to understand these time-dependent microscopic processes. Some of these applications will be illustrated by recent results performed at synchrotrons. New powerful x-ray sources now under construction offer the opportunity to apply innovative approaches in time-resolved work

  10. High Brightness, Laser-Driven X-ray Source for Nanoscale Metrology and Femtosecond Dynamics

    Energy Technology Data Exchange (ETDEWEB)

    Siders, C W; Crane, J K; Semenov, V; Betts, S; Kozioziemski, B; Wharton, K; Wilks, S; Barbee, T; Stuart, B; Kim, D E; An, J; Barty, C

    2007-02-26

    This project developed and demonstrated a new, bright, ultrafast x-ray source based upon laser-driven K-alpha generation, which can produce an x-ray flux 10 to 100 times greater than current microfocus x-ray tubes. The short-pulse (sub-picosecond) duration of this x-ray source also makes it ideal for observing time-resolved dynamics of atomic motion in solids and thin films.

  11. Laser-produced X-ray sources

    International Nuclear Information System (INIS)

    Hudson, L.T.; Seely, J.F.

    2010-01-01

    A formidable array of advanced laser systems are emerging that produce extreme states of light and matter. By irradiating solid and gaseous targets with lasers of increasing energy densities, new physical regimes of radiation effects are being explored for the first time in controlled laboratory settings. One result that is being accomplished or pursued using a variety of techniques, is the realization of novel sources of X-rays with unprecedented characteristics and light-matter interactions, the mechanisms of which are in many cases still being elucidated. Examples include the megajoule class of laser-produced plasmas designed in pursuit of alternative-energy and security applications and the petawatt class of lasers used for fast ignition and X-ray radiographic applications such as medical imaging and real-time imaging of plasma hydrodynamics. As these technologies mature, increased emphasis will need to be placed on advanced instrumentation and diagnostic metrology to characterize the spectra, time structure, and absolute brightness of X-rays emitted by these unconventional sources. Such customized and absolutely calibrated measurement tools will serve as an enabling technology that can help in assessing the overall system performance and progress, as well as identification of the underlying interaction mechanisms of interest to basic and applied strong-field and high-energy-density science.

  12. X-ray laser research at Palaiseau

    International Nuclear Information System (INIS)

    Jaegle, P.; Jamelot, G.; Carillon, A.; Klisnick, A.; Paris-11 Univ., 91 - Orsay

    1986-01-01

    We present the soft X-ray laser experiments performed at Greco ''Interaction Laser-Matiere'' (Palaiseau). They are mainly concerned with lithium-like ions of aluminium in plasmas produced by 1.06 μ Nd-laser. We describe the experimental set-up which performs time-dependent gain measurements. We report results showing a gain-length product of 2 - 2.5 for the 3d - 5f line at 105.7 A. Comparison is made between experiment and computational model. The possible limiting role of radiation trapping for long plasma column is discussed. We present the future projects regarding larger gains and new wavelengths

  13. Gas detectors for x-ray lasers

    International Nuclear Information System (INIS)

    Tiedtke, K.; Feldhaus, J.; Hahn, U.; Jastrow, U.; Nunez, T.; Tschentscher, T.; Bobashev, S. V.; Sorokin, A. A.; Hastings, J. B.; Moeller, S.; Cibik, L.; Gottwald, A.; Hoehl, A.; Kroth, U.; Krumrey, M.; Schoeppe, H.; Ulm, G.; Richter, M.

    2008-01-01

    We have developed different types of photodetectors that are based on the photoionization of a gas at a low target density. The almost transparent devices were optimized and tested for online photon diagnostics at current and future x-ray free-electron laser facilities on a shot-to-shot basis with a temporal resolution of better than 100 ns. Characterization and calibration measurements were performed in the laboratory of the Physikalisch-Technische Bundesanstalt at the electron storage ring BESSY II in Berlin. As a result, measurement uncertainties of better than 10% for the photon-pulse energy and below 20 μm for the photon-beam position were achieved at the Free-electron LASer in Hamburg (FLASH). An upgrade for the detection of hard x-rays was tested at the Sub-Picosecond Photon Source in Stanford

  14. Gas detectors for x-ray lasers

    Science.gov (United States)

    Tiedtke, K.; Feldhaus, J.; Hahn, U.; Jastrow, U.; Nunez, T.; Tschentscher, T.; Bobashev, S. V.; Sorokin, A. A.; Hastings, J. B.; Möller, S.; Cibik, L.; Gottwald, A.; Hoehl, A.; Kroth, U.; Krumrey, M.; Schöppe, H.; Ulm, G.; Richter, M.

    2008-05-01

    We have developed different types of photodetectors that are based on the photoionization of a gas at a low target density. The almost transparent devices were optimized and tested for online photon diagnostics at current and future x-ray free-electron laser facilities on a shot-to-shot basis with a temporal resolution of better than 100 ns. Characterization and calibration measurements were performed in the laboratory of the Physikalisch-Technische Bundesanstalt at the electron storage ring BESSY II in Berlin. As a result, measurement uncertainties of better than 10% for the photon-pulse energy and below 20 μm for the photon-beam position were achieved at the Free-electron LASer in Hamburg (FLASH). An upgrade for the detection of hard x-rays was tested at the Sub-Picosecond Photon Source in Stanford.

  15. Ultrafast Structural Dynamics in InSb Probed by Time-Resolved X-Ray Diffraction

    International Nuclear Information System (INIS)

    Chin, A.H.; Shank, C.V.; Chin, A.H.; Schoenlein, R.W.; Shank, C.V.; Glover, T.E.; Leemans, W.P.; Balling, P.

    1999-01-01

    Ultrafast structural dynamics in laser-perturbed InSb are studied using time-resolved x-ray diffraction with a novel femtosecond x-ray source. We report the first observation of a delay in the onset of lattice expansion, which we attribute to energy relaxation processes and lattice strain propagation. In addition, we observe direct indications of ultrafast disordering on a subpicosecond time scale. copyright 1999 The American Physical Society

  16. Frequency filter of seed x-ray by use of x-ray laser medium. Toward the generation of the temporally coherent x-ray laser

    International Nuclear Information System (INIS)

    Hasegawa, Noboru; Kawachi, Tetsuya; Kishimoto, Maki; Sukegawa, Kouta; Tanaka, Momoko; Ochi, Yoshihiro; Nishikino, Masaharu; Nagashima, Keisuke; Kato, Yoshiaki; Renzhong, Tai

    2009-01-01

    We evaluate the characteristics of a higher-order harmonics light as a seed X-ray amplified through a laser-produced X-ray amplifier. The narrow spectral bandwidth of the X-ray amplifier works as the frequency filter of the seed X-ray, resulting in that only the temporally coherent X-ray is amplified. Experimental investigation using the 29th-order harmonic light of the Ti:sapphire laser at a wavelength of 26.9 nm together with a neon-like manganese X-ray laser medium shows evident spectral narrowing of the seed X-ray and amplification without serious diffraction effects on the propagation of the amplified X-ray beam. This implies that the present combination is potential to realize temporally coherent X-ray lasers, with an expected duration of approximately 400 fs. (author)

  17. Diagnostics for an XUV/soft x-ray laser

    International Nuclear Information System (INIS)

    Kauffman, R.L.; Matthews, D.L.; Ceglio, N.; Medecki, H.

    1984-01-01

    We have begun investigating the production of an XUV/soft x-ray laser, using our high-powered glass lasers as drivers. A major diagnostic for lasing is the measure of the absolute power produced in the lasing line. I have developed a spectrograph to time-resolved lasing lines in the energy range from 50 eV to greater than 200 eV. the spectrograph combines a transmission grating and x-ray streak camera to produce a flat field instrument. A cylindrical mirror is used in front of the grating to image the source and act as a collecting optic. The efficiency of the components is calibrated so that absolute intensities can be measured. I will compare the performance of this instrument with reflection grating systems. I will also discuss planned improvements to the system which should increase total throughput, image quality, and resolving power

  18. Resolve Instrument on X-ray Astronomy Recovery Mission (XARM)

    Science.gov (United States)

    Ishisaki, Y.; Ezoe, Y.; Yamada, S.; Ichinohe, Y.; Fujimoto, R.; Takei, Y.; Yasuda, S.; Ishida, M.; Yamasaki, N. Y.; Maeda, Y.; Tsujimoto, M.; Iizuka, R.; Koyama, S.; Noda, H.; Tamagawa, T.; Sawada, M.; Sato, K.; Kitamoto, S.; Hoshino, A.; Brown, G. V.; Eckart, M. E.; Hayashi, T.; Kelley, R. L.; Kilbourne, C. A.; Leutenegger, M. A.; Mori, H.; Okajima, T.; Porter, F. S.; Soong, Y.; McCammon, D.; Szymkowiak, A. E.

    2018-04-01

    The X-ray Astronomy Recovery Mission (XARM) is a recovery mission of ASTRO-H/Hitomi, which is expected to be launched in Japanese Fiscal Year of 2020 at the earliest. The Resolve instrument on XARM consists of an array of 6 × 6 silicon-thermistor microcalorimeters cooled down to 50 mK and a high-throughput X-ray mirror assembly with the focal length of 5.6 m. Hitomi was launched into orbit in February 2016 and observed several celestial objects, although the operation of Hitomi was terminated in April 2016. The soft X-ray spectrometer (SXS) on Hitomi demonstrated high-resolution X-ray spectroscopy of 5 eV FWHM in orbit for most of the pixels. The Resolve instrument is planned to mostly be a copy of the Hitomi SXS and soft X-ray telescope designs, though several changes are planned based on the lessons learned from Hitomi. We report a brief summary of the SXS performance and the status of the Resolve instrument.

  19. Enhanced brightness x-ray lasers

    International Nuclear Information System (INIS)

    Wan, A.S.; Cauble, R.C.; Da Silva, L.B.; Moreno, J.C.; Nilsen, J.

    1994-09-01

    We are developing short-pulsed, enhanced-brightness, and coherent x-ray lasers (XRLs) for applications in areas such as plasma imaging. In a traveling wave pump setup the optical laser creating the XRL plasma sweeps along the lasant axis at the same speed as the x-rays. This technique becomes increasingly important as the target length increases and the gain duration shortens. An order of magnitude increase in output energy was measured with vs without traveling wave pump. Using multiple pulse techniques and multilayer mirrors to inject the output of one pulse back into the plasma formed by a later pulse we have begun to develop the x-ray analog of a multi-pass amplifler. The use of multiple pulses separated by as much as 1.6 ns reduces multilayer mirror damage. This injection technique is demonstrated by imaging the near-field emission profiles of the XRL. The addition of multilayer beamsplitter will allow us to effectively produce a soft XRL cavity

  20. An instrument for in situ time-resolved X-ray imaging and diffraction of laser powder bed fusion additive manufacturing processes

    Science.gov (United States)

    Calta, Nicholas P.; Wang, Jenny; Kiss, Andrew M.; Martin, Aiden A.; Depond, Philip J.; Guss, Gabriel M.; Thampy, Vivek; Fong, Anthony Y.; Weker, Johanna Nelson; Stone, Kevin H.; Tassone, Christopher J.; Kramer, Matthew J.; Toney, Michael F.; Van Buuren, Anthony; Matthews, Manyalibo J.

    2018-05-01

    In situ X-ray-based measurements of the laser powder bed fusion (LPBF) additive manufacturing process produce unique data for model validation and improved process understanding. Synchrotron X-ray imaging and diffraction provide high resolution, bulk sensitive information with sufficient sampling rates to probe melt pool dynamics as well as phase and microstructure evolution. Here, we describe a laboratory-scale LPBF test bed designed to accommodate diffraction and imaging experiments at a synchrotron X-ray source during LPBF operation. We also present experimental results using Ti-6Al-4V, a widely used aerospace alloy, as a model system. Both imaging and diffraction experiments were carried out at the Stanford Synchrotron Radiation Lightsource. Melt pool dynamics were imaged at frame rates up to 4 kHz with a ˜1.1 μm effective pixel size and revealed the formation of keyhole pores along the melt track due to vapor recoil forces. Diffraction experiments at sampling rates of 1 kHz captured phase evolution and lattice contraction during the rapid cooling present in LPBF within a ˜50 × 100 μm area. We also discuss the utility of these measurements for model validation and process improvement.

  1. 14th International Conference on X-Ray Lasers

    CERN Document Server

    Menoni, Carmen; Marconi, Mario

    2016-01-01

    These proceedings comprise invited and contributed papers presented at the 14th International Conference on X-Ray Lasers (ICXRL 2014). This conference is part of a continuing series dedicated to recent developments and applications of x-ray lasers and other coherent x-ray sources with attention to supporting technologies and instrumentation. New results in the generation of intense, coherent x-rays and progress toward practical devices and their applications in numerous fields are reported. Areas of research in plasma-based x-ray lasers, 4th generation accelerator-based sources and higher harmonic generation, and other x-ray generation schemes are covered.  The scope of ICXRL 2014 included, but was not limited to: Laser-pumped X-ray lasers Discharge excitation and other X-ray laser pumping methods Injection/seeding of X-ray amplifiers New lasing transitions and novel X-ray laser schemes High Harmonic sources-Free-electron laser generation in the XUV and X-ray range Novel schemes for coherent XUV and X-ray ge...

  2. X-ray Free-electron Lasers

    Energy Technology Data Exchange (ETDEWEB)

    Feldhaus, J.; /DESY; Arthur, J.; Hastings, J.B.; /SLAC

    2007-02-23

    In a free-electron laser (FEL) the lasing medium is a high-energy beam of electrons flying with relativistic speed through a periodic magnetic field. The interaction between the synchrotron radiation that is produced and the electrons in the beam induces a periodic bunching of the electrons, greatly increasing the intensity of radiation produced at a particular wavelength. Depending only on a phase match between the electron energy and the magnetic period, the wavelength of the FEL radiation can be continuously tuned within a wide spectral range. The FEL concept can be adapted to produce radiation wavelengths from millimeters to Angstroms, and can in principle produce hard x-ray beams with unprecedented peak brightness, exceeding that of the brightest synchrotron source by ten orders of magnitude or more. This paper focuses on short-wavelength FELs. It reviews the physics and characteristic properties of single-pass FELs, as well as current technical developments aiming for fully coherent x-ray radiation pulses with pulse durations in the 100 fs to 100 as range. First experimental results at wavelengths around 100 nm and examples of scientific applications planned on the new, emerging x-ray FEL facilities are presented.

  3. Direct observation of ultrafast atomic motion using time-resolved X-ray diffraction

    Energy Technology Data Exchange (ETDEWEB)

    Shymanovich, U.

    2007-11-13

    This thesis is dedicated to the study of the atomic motion in laser irradiated solids on a picosecond to subpicosecond time-scale using the time-resolved X-ray diffraction technique. In the second chapter, the laser system, the laser-plasma based X-ray source and the experimental setup for optical pump / X-ray probe measurements were presented. Chapter 3 is devoted to the characterization and comparison of different types of X-ray optics. Chapter 4 presented the time-resolved X-ray diffraction experiments performed for this thesis. The first two sections of this chapter discuss the measurements of initially unexpected strain-induced transient changes of the integrated reflectivity of the X-ray probe beam. The elimination of the strain-induced transient changes of the integrated reflectivity represented an important prerequisite to perform the study of lattice heating in Germanium after femtosecond optical excitation by measuring the transient Debye-Waller effect. The third section describes the investigations of acoustic waves upon ultrafast optical excitation and discusses the two different pressure contributions driving them: the thermal and the electronic ones. (orig.)

  4. Direct observation of ultrafast atomic motion using time-resolved X-ray diffraction

    International Nuclear Information System (INIS)

    Shymanovich, U.

    2007-01-01

    This thesis is dedicated to the study of the atomic motion in laser irradiated solids on a picosecond to subpicosecond time-scale using the time-resolved X-ray diffraction technique. In the second chapter, the laser system, the laser-plasma based X-ray source and the experimental setup for optical pump / X-ray probe measurements were presented. Chapter 3 is devoted to the characterization and comparison of different types of X-ray optics. Chapter 4 presented the time-resolved X-ray diffraction experiments performed for this thesis. The first two sections of this chapter discuss the measurements of initially unexpected strain-induced transient changes of the integrated reflectivity of the X-ray probe beam. The elimination of the strain-induced transient changes of the integrated reflectivity represented an important prerequisite to perform the study of lattice heating in Germanium after femtosecond optical excitation by measuring the transient Debye-Waller effect. The third section describes the investigations of acoustic waves upon ultrafast optical excitation and discusses the two different pressure contributions driving them: the thermal and the electronic ones. (orig.)

  5. X-ray lasers for structural and dynamic biology

    International Nuclear Information System (INIS)

    Spence, J C H; Weierstall, U; Chapman, H N

    2012-01-01

    Research opportunities and techniques are reviewed for the application of hard x-ray pulsed free-electron lasers (XFEL) to structural biology. These include the imaging of protein nanocrystals, single particles such as viruses, pump–probe experiments for time-resolved nanocrystallography, and snapshot wide-angle x-ray scattering (WAXS) from molecules in solution. The use of femtosecond exposure times, rather than freezing of samples, as a means of minimizing radiation damage is shown to open up new opportunities for the molecular imaging of biochemical reactions at room temperature in solution. This is possible using a ‘diffract-and-destroy’ mode in which the incident pulse terminates before radiation damage begins. Methods for delivering hundreds of hydrated bioparticles per second (in random orientations) to a pulsed x-ray beam are described. New data analysis approaches are outlined for the correlated fluctuations in fast WAXS, for protein nanocrystals just a few molecules on a side, and for the continuous x-ray scattering from a single virus. Methods for determining the orientation of a molecule from its diffraction pattern are reviewed. Methods for the preparation of protein nanocrystals are also reviewed. New opportunities for solving the phase problem for XFEL data are outlined. A summary of the latest results is given, which now extend to atomic resolution for nanocrystals. Possibilities for time-resolved chemistry using fast WAXS (solution scattering) from mixtures is reviewed, toward the general goal of making molecular movies of biochemical processes. (key issues reviews)

  6. Table-top instrumentation for time-resolved luminescence spectroscopy of solids excited by nanosecond pulse of soft X-ray source and/or UV laser

    International Nuclear Information System (INIS)

    Bruza, Petr; Fidler, Vlastimil; Nikl, Martin

    2011-01-01

    The practical applicability of the rare-earth doped scintillators in high-speed detectors is limited by the slow decay components in the temporal response of a scintillator. The study of origin and properties of material defects that induce the slow decay components is of major importance for the development of new scintillation materials. We present a table-top, time-domain UV-VIS luminescence spectrometer, featuring extended time and input sensitivity ranges and two excitation sources. The combination of both soft X-ray/XUV and UV excitation source allows the comparative measurements of luminescence spectra and decay kinetics of scintillators to be performed under the same experimental conditions. The luminescence of emission centers of a doped scintillator can be induced by conventional N 2 laser pulse, while the complete scintillation process can be initiated by a soft X-ray/XUV pulse excitation from the laser-produced plasma in gas puff target of 4 ns duration. In order to demonstrate the spectrometer, the UV-VIS luminescence spectra and decay kinetics of cerium doped Lu 3 Al 5 O 12 single crystal (LuAG:Ce) scintillator excited by XUV and UV radiation were acquired. Luminescence of the doped Ce 3+ ions was studied under 2.88 nm (430 eV) XUV excitation from the laser-produced nitrogen plasma, and compared with the luminescence under 337 nm (3.68 eV) UV excitation from nitrogen laser. In the former case the excitation energy is deposited in the LuAG host, while in the latter the 4f-5d 2 transition of Ce 3+ is directly excited. Furthermore, YAG:Ce and LuAG:Ce single crystals luminescence decay profiles are compared and discussed.

  7. Chemical bond activation observed with an x-ray laser

    International Nuclear Information System (INIS)

    Beye, Martin; Öberg, Henrik; Xin, Hongliang

    2016-01-01

    The concept of bonding and anti-bonding orbitals is fundamental in chemistry. The population of those orbitals and the energetic difference between the two reflect the strength of the bonding interaction. Weakening the bond is expected to reduce this energetic splitting, but the transient character of bond-activation has so far prohibited direct experimental access. Lastly, we apply time-resolved soft X-ray spectroscopy at a free-electron laser to directly observe the decreased bonding–anti-bonding splitting following bond-activation using an ultra short optical laser pulse.

  8. Time-Resolved Hard X-Ray Spectrometer

    International Nuclear Information System (INIS)

    Kenneth Moya; Ian McKennaa; Thomas Keenana; Michael Cuneob

    2007-01-01

    Wired array studies are being conducted at the SNL Z accelerator to maximize the x-ray generation for inertial confinement fusion targets and high energy density physics experiments. An integral component of these studies is the characterization of the time-resolved spectral content of the x-rays. Due to potential spatial anisotropy in the emitted radiation, it is also critical to diagnose the time-evolved spectral content in a space-resolved manner. To accomplish these two measurement goals, we developed an x-ray spectrometer using a set of high-speed detectors (silicon PIN diodes) with a collimated field-of-view that converged on a 1-cm-diameter spot at the pinch axis. Spectral discrimination is achieved by placing high Z absorbers in front of these detectors. We built two spectrometers to permit simultaneous different angular views of the emitted radiation. Spectral data have been acquired from recent Z shots for the radial and polar views. UNSPEC1 has been adapted to analyze and unfold the measured data to reconstruct the x-ray spectrum. The unfold operator code, UFO2, is being adapted for a more comprehensive spectral unfolding treatment

  9. X-ray lasers: from star wars to benchtop systems

    International Nuclear Information System (INIS)

    Kuba, J.; Limpouch, J.; Drska, L.

    2005-01-01

    The paper is structured as follows: The principle of X-ray lasers; The transient scheme - an X-ray laser (maybe) on a laboratory bench; The experimental parameters of transient lasers show promise; and The nuclear gamma laser is one of the feasible pathways. (P.A.)

  10. X-ray laser studies at LLE

    International Nuclear Information System (INIS)

    Yaakobi, B.; Boehly, T.; Audebert, P.; Epstein, R.; Boswell, B.; Richardson, M.C.; Soures, J.M.; Shvarts, D.

    1988-01-01

    New target geometries for collisional excitation X-ray laser experiments (in nickel) were proposed, analyzed, and experimentally studied on the GDL laser. Experiments using a short line focus lens with new target geometries showed general agreement with predictions. The new geometries are designed to yield a higher gain and reduced refraction due to 1) a higher plasma density, 2) a wider lateral density profile, and 3) a concave lateral density profile. These new geometries were a) two parallel exploding (thin) foils, irradiated from one side only, b) two ablating (thick) foils, one of which is irradiated on its inner face, and c) an exploding foil in front of an ablating foil, irradiated by a single laser beam incident on the thin foil. The experiments with a long line focus are in progress. The intensity ratio of Ne-like and F-like Ni lines is used to deduce the temperature, and these results together with the absolute intensity yields the density profile. The results show improvement achieved with the new target geometries: the density is higher (leading to a higher gain), and the concave density profile results in collimation rather than divergence of the X-ray laser beam. Theoretical developments included development of a ray-tracing code for an amplifying medium of varying (e.g., collimating) lateral density profile (results using this code are shown for convex as well as concave lateral density profiles) and prediction of high gain on new type transitions in neonlike ions, involving the excitation of an inner (2s) electron

  11. Development of short pulse laser pumped x-ray lasers

    International Nuclear Information System (INIS)

    Dunn, J; Osterheld, A L; Hunter, J R; Shlyaptsev, V N

    2000-01-01

    X-ray lasers have been extensively studied around the world since the first laboratory demonstration on the Novette laser at LLNL in 1984 [l]. The characteristic properties of short wavelength, high monochromaticity, collimation and coherence make x-ray lasers useful for various applications. These include demonstrations of biological imaging within the water window, interferometry of laser plasmas and radiography of laser-heated surfaces. One of the critical issues has been the high power pump required to produce the inversion. The power scaling as a function of x-ray laser wavelength follows a -k4 to law. The shortest x-ray laser wavelength of ∼ 35 (angstrom) demonstrated for Ni-like All was at the limit of Nova laser capabilities. By requiring large, high power lasers such as Nova, the shot rate and total number of shots available have limited the rapid development of x-ray lasers and applications. In fact over the last fifteen years the main thrust has been to develop more efficient, higher repetition rate x-ray lasers that can be readily scaled to shorter wavelengths. The recent state of progress in the field can be found in references. The objective of the project was to develop a soft x-ray laser (XRL) pumped by a short pulse laser of a few joules. In effect to demonstrate a robust, worlung tabletop x-ray laser at LLNL for the first time. The transient collisional scheme as proposed by Shlyaptsev et al [8, 9] was the candidate x-ray laser for study. The successful endeavour of any scientific investigation is often based upon prudent early decisions and the choice of this scheme was both sound and fruitful. It had been demonstrated very recently for Ne-like Ti at 326 A using a small tabletop laser [10] but had not yet reached its full potential. We chose this scheme for several reasons: (a) it was a collisional-type x-ray laser which has been historically the most robust; (b) it had the promise of high efficiency and low energy threshold for lasing; (c) the

  12. Time-resolved X-ray spectroscopies of chemical systems: New perspectives

    Directory of Open Access Journals (Sweden)

    Majed Chergui

    2016-05-01

    Full Text Available The past 3–5 years have witnessed a dramatic increase in the number of time-resolved X-ray spectroscopic studies, mainly driven by novel technical and methodological developments. The latter include (i the high repetition rate optical pump/X-ray probe studies, which have greatly boosted the signal-to-noise ratio for picosecond (ps X-ray absorption spectroscopy studies, while enabling ps X-ray emission spectroscopy (XES at synchrotrons; (ii the X-ray free electron lasers (XFELs are a game changer and have allowed the first femtosecond (fs XES and resonant inelastic X-ray scattering experiments to be carried out; (iii XFELs are also opening the road to the development of non-linear X-ray methods. In this perspective, I will mainly focus on the most recent technical developments and briefly address some examples of scientific questions that have been addressed thanks to them. I will look at the novel opportunities in the horizon.

  13. X-ray emission from stainless steel foils irradiated by femtosecond petawatt laser pulses

    Science.gov (United States)

    Alkhimova, M. A.; Faenov, A. Ya; Pikuz, T. A.; Skobelev, I. Yu; Pikuz, S. A.; Nishiuchi, M.; Sakaki, H.; Pirozhkov, A. S.; Sagisaka, S.; Dover, N. P.; Kondo, Ko; Ogura, K.; Fukuda, Y.; Kiriyama, H.; Esirkepov, T.; Bulanov, S. V.; Andreev, A.; Kando, M.; Zhidkov, A.; Nishitani, K.; Miyahara, T.; Watanabe, Y.; Kodama, R.; Kondo, K.

    2018-01-01

    We report about nonlinear growth of x-ray emission intensity emitted from plasma generated by femtosecond petawatt laser pulses irradiating stainless steel foils. X-ray emission intensity increases as ˜ I 4.5 with laser intensity I on a target. High spectrally resolved x-ray emission from front and rear surfaces of 5 μm thickness stainless steel targets were obtained at the wavelength range 1.7-2.1 Å, for the first time in experiments at femtosecond petawatt laser facility J-KAREN-P. Total intensity of front x-ray spectra three times dominates to rear side spectra for maximum laser intensity I ≈ 3.2×1021 W/cm2. Growth of x-ray emission is mostly determined by contribution of bremsstrahlung radiation that allowed estimating bulk electron plasma temperature for various magnitude of laser intensity on target.

  14. Ultrafast, laser-based, x-ray science: the dawn of atomic-scale cinematography

    International Nuclear Information System (INIS)

    Barty, C.P.J.

    2000-01-01

    The characteristics of ultrafast chirped pulse amplification systems are reviewed. Application of ultrafast chirped pulse amplification to the generation of femtosecond, incoherent, 8-keV line radiation is outlined and the use of femtosecond laser-based, x-rays for novel time-resolved diffraction studies of crystalline dynamics with sub-picosecond temporal resolution and sub-picometer spatial resolution is reviewed in detail. Possible extensions of laser-based, x-ray technology and evaluation of alternative x-ray approaches for time-resolved studies of the atomic scale dynamics are given. (author)

  15. Ultrafast, laser-based, x-ray science: the dawn of atomic-scale cinematography

    Energy Technology Data Exchange (ETDEWEB)

    Barty, C.P.J. [University of California, Department of Applied Mechanics and Engineering Science, Urey Hall, Mali Code 0339, San Diego, La Jolla, CA (United States)

    2000-03-01

    The characteristics of ultrafast chirped pulse amplification systems are reviewed. Application of ultrafast chirped pulse amplification to the generation of femtosecond, incoherent, 8-keV line radiation is outlined and the use of femtosecond laser-based, x-rays for novel time-resolved diffraction studies of crystalline dynamics with sub-picosecond temporal resolution and sub-picometer spatial resolution is reviewed in detail. Possible extensions of laser-based, x-ray technology and evaluation of alternative x-ray approaches for time-resolved studies of the atomic scale dynamics are given. (author)

  16. Spatially resolved density and ionization measurements of shocked foams using x-ray fluorescence

    Energy Technology Data Exchange (ETDEWEB)

    MacDonald, M. J.; Keiter, P. A.; Montgomery, D. S.; Scott, H. A.; Biener, M. M.; Fein, J. R.; Fournier, K. B.; Gamboa, E. J.; Kemp, G. E.; Klein, S. R.; Kuranz, C. C.; LeFevre, H. J.; Manuel, M. J. -E.; Wan, W. C.; Drake, R. P.

    2016-09-28

    We present experiments at the Trident laser facility demonstrating the use of x-ray fluorescence (XRF) to simultaneously measure density, ionization state populations, and electron temperature in shocked foams. An imaging x-ray spectrometer obtained spatially resolved measurements of Ti K-α emission. Density profiles were measured from K-α intensity. Ti ionization state distributions and electron temperatures were inferred by fitting K-α spectra to spectra from CRETIN simulations. This work shows that XRF provides a powerful tool to complement other diagnostics to make equation of state measurements of shocked materials containing a suitable tracer element.

  17. Time Resolved X-Ray Scattering of molecules in Solution

    DEFF Research Database (Denmark)

    Brandt van Driel, Tim

    The dissertation describes the use of Time-Resolved X-ray Diffuse Scattering (TR-XDS) to study photo-induced structural changes in molecules in solution. The application of the technique is exemplified with experiments on two bimetallic molecules. The main focus is on the data-flow and process......)42+ obtained at European Synchrotron Radiation Facility (ESRF) are presented to exemplify TR-XDS at synchrotrons. Similarly, measurements on Ir2(dimen)42+ are used to show the XFEL data-flow and how it deviates from the prior. A method to identify and account for systematic fluctuations...

  18. Using acoustic levitation in synchrotron based laser pump hard x-ray probe experiments

    Science.gov (United States)

    Hu, Bin; Lerch, Jason; Suthar, Kamlesh; Dichiara, Anthony

    Acoustic levitation provides a platform to trap and hold a small amount of material by using standing pressure waves without a container. The technique has a potential to be used for laser pump x-ray probe experiments; x-ray scattering and laser distortion from the container can be avoided, sample consumption can be minimized, and unwanted chemistry that may occur at the container interface can be avoided. The method has been used at synchrotron sources for studying protein and pharmaceutical solutions using x-ray diffraction (XRD) and small angle x-ray scattering (SAXS). However, pump-probe experiments require homogeneously excited samples, smaller than the absorption depth of the material that must be held stably at the intersection of both the laser and x-ray beams. We discuss 1) the role of oscillations in acoustic levitation and the optimal acoustic trapping conditions for x-ray/laser experiments, 2) opportunities to automate acoustic levitation for fast sample loading and manipulation, and 3) our experimental results using SAXS to monitor laser induced thermal expansion in gold nanoparticles solution. We also performed Finite Element Analysis to optimize the trapping performance and stability of droplets ranging from 0.4 mm to 2 mm. Our early x-ray/laser demonstrated the potential of the technique for time-resolved X-ray science.

  19. High resolution time- and 2-dimensional space-resolved x-ray imaging of plasmas at NOVA

    International Nuclear Information System (INIS)

    Landen, O.L.

    1992-01-01

    A streaked multiple pinhole camera technique, first used by P. Choi et al. to record time- and 2-D space-resolved soft X-ray images of plasma pinches, has been implemented on laser plasmas at NOVA. The instrument is particularly useful for time-resolved imaging of small sources ( 2.5 key imaging, complementing the existing 1--3 key streaked X-ray microscope capabilities at NOVA

  20. Characterization and modeling of soft x-ray lasers

    International Nuclear Information System (INIS)

    Wan, A.S.; Cauble, R.; Celliers, P.; DaSilva, L.B.; Libby, S.B.; London, R.A.; Nilsen, J.; Moreno, J.C.; Weber, F.

    1995-01-01

    This paper describes our theoretical, numerical, and experimental development of short-pulse-duration, high brightness, and enhanced coherence x-ray lasers (XRLs) as sources suitable for applications as imaging diagnostics for laser plasmas

  1. Time-resolved X-ray photoelectron spectroscopy techniques for the study of interfacial charge dynamics

    Energy Technology Data Exchange (ETDEWEB)

    Neppl, Stefan, E-mail: sneppl@lbl.gov; Gessner, Oliver

    2015-04-15

    Highlights: • Ultrafast interfacial charge transfer is probed with atomic site specificity. • Femtosecond X-ray photoelectron spectroscopy using a free electron laser. • Efficient and flexible picosecond X-ray photoelectron pump–probe scheme using synchrotron radiation. - Abstract: X-ray photoelectron spectroscopy (XPS) is one of the most powerful techniques to quantitatively analyze the chemical composition and electronic structure of surfaces and interfaces in a non-destructive fashion. Extending this technique into the time domain has the exciting potential to shed new light on electronic and chemical dynamics at surfaces by revealing transient charge configurations with element- and site-specificity. Here, we describe prospects and challenges that are associated with the implementation of picosecond and femtosecond time-resolved X-ray photoelectron spectroscopy at third-generation synchrotrons and X-ray free-electron lasers, respectively. In particular, we discuss a series of laser-pump/X-ray-probe photoemission experiments performed on semiconductor surfaces, molecule-semiconductor interfaces, and films of semiconductor nanoparticles that demonstrate the high sensitivity of time-resolved XPS to light-induced charge carrier generation, diffusion and recombination within the space charge layers of these materials. Employing the showcase example of photo-induced electronic dynamics in a dye-sensitized semiconductor system, we highlight the unique possibility to probe heterogeneous charge transfer dynamics from both sides of an interface, i.e., from the perspective of the molecular electron donor and the semiconductor acceptor, simultaneously. Such capabilities will be crucial to improve our microscopic understanding of interfacial charge redistribution and associated chemical dynamics, which are at the heart of emerging energy conversion, solar fuel generation, and energy storage technologies.

  2. Structural enzymology using X-ray free electron lasers

    Directory of Open Access Journals (Sweden)

    Christopher Kupitz

    2017-07-01

    Full Text Available Mix-and-inject serial crystallography (MISC is a technique designed to image enzyme catalyzed reactions in which small protein crystals are mixed with a substrate just prior to being probed by an X-ray pulse. This approach offers several advantages over flow cell studies. It provides (i room temperature structures at near atomic resolution, (ii time resolution ranging from microseconds to seconds, and (iii convenient reaction initiation. It outruns radiation damage by using femtosecond X-ray pulses allowing damage and chemistry to be separated. Here, we demonstrate that MISC is feasible at an X-ray free electron laser by studying the reaction of M. tuberculosis ß-lactamase microcrystals with ceftriaxone antibiotic solution. Electron density maps of the apo-ß-lactamase and of the ceftriaxone bound form were obtained at 2.8 Å and 2.4 Å resolution, respectively. These results pave the way to study cyclic and non-cyclic reactions and represent a new field of time-resolved structural dynamics for numerous substrate-triggered biological reactions.

  3. X-ray diagnostics for laser matter interaction experiments

    International Nuclear Information System (INIS)

    Troussel, Ph.

    2000-01-01

    Advances in the field of laser-driven inertially confined thermonuclear fusion research since the early 1990's are reviewed. It covers the experimental techniques used to study the interaction of laser radiation with matter and high density plasma. A high performance instrumentation (diagnostics) for observation of X radiation (from a few eV to a few keV) will be required to understand the physical processes involved in the interaction. This paper is a three-part: first part, describes diagnostics metrology realized around different X-ray sources (synchrotron, laser plasma...); a second part, synthesizes theoretical and experimental X-ray optics studies and show the interest for direct applications as X-ray spectroscopy and X-ray imaging around laser-produced plasma; a third part, is a review of high resolution X-ray imaging, performances of these optical system were summarized. (author)

  4. Lasers, extreme UV and soft X-ray

    Energy Technology Data Exchange (ETDEWEB)

    Nilsen, Joseph [Lawrence Livermore National Lab. (LLNL), Livermore, CA (United States)

    2015-09-20

    Three decades ago, large ICF lasers that occupied entire buildings were used as the energy sources to drive the first X-ray lasers. Today X-ray lasers are tabletop, spatially coherent, high-repetition rate lasers that enable many of the standard optical techniques such as interferometry to be extended to the soft X-ray regime between wavelengths of 10 and 50 nm. Over the last decade X-ray laser performance has been improved by the use of the grazing incidence geometry, diode-pumped solid-state lasers, and seeding techniques. The dominant X-ray laser schemes are the monopole collisional excitation lasers either driven by chirped pulse amplification (CPA) laser systems or capillary discharge. The CPA systems drive lasing in neon-like or nickel-like ions, typically in the 10 – 30 nm range, while the capillary system works best for neon-like argon at 46.9 nm. Most researchers use nickel-like ion lasers near 14 nm because they are well matched to the Mo:Si multilayer mirrors that have peak reflectivity near 13 nm and are used in many applications. As a result, the last decade has seen the birth of the X-ray free electron laser (XFEL) that can reach wavelengths down to 0.15 nm and the inner-shell Ne laser at 1.46 nm.

  5. Development of small scale soft x-ray lasers

    International Nuclear Information System (INIS)

    Kim, D.; Suckewer, S.; Princeton Univ., NJ; Skinner, C.H.; Voorhees, D.

    1991-05-01

    At present rapid progress is being made in the application of soft x-ray lasers to fields such as microscopy and microlithography. A critical factor in the range of suitable applications is the scale and hence cost of the soft x-ray lasers. At Princeton, gain at 183 angstrom has been obtained with relatively low pump laser energies (as low as 6J) in a ''portable'' small-scale soft x-ray laser system. We will also discuss aspects of data interpretation and pitfalls to be avoided in measurements of gain in such systems. 14 refs., 7 figs

  6. Soft X-Ray amplification in laser plasmas

    International Nuclear Information System (INIS)

    Louis-Jacquet, M.

    1988-01-01

    The principles, experiments and theoretical models of soft x-ray, amplification, produced in laser plasmas, are studied. In the discussion of the principles, the laser plasma medium, the definition of the gain, the population inversions, saturation and superradiance are described. The results concerning recombination and collisional excitation experiments, as well as experimental devices are shown. A complete physical simulation to design and interpret x-ray laser experiments is given. Applications of x-ray lasers in grating production techniques, in contact microscopy and holography are considered

  7. X-ray laser '' oscillator-amplifier'' experiments

    International Nuclear Information System (INIS)

    Shimkaveg, G.M.; Carter, M.R.; Young, B.K.F.; Walling, R.S.; Osterheld, A.L.; Trebes, J.E.; London, R.A.; Ratowsky, R.P.; Stewart, R.E.; Craxton, R.S.

    1993-01-01

    We present results from experiments directed toward increasing the degree of transverse coherence in x-ray laser beams. We have concentrated on the neon-like yttrium (Z=39) collisionally-pumped x-ray laser as the test system for these studies because of its unique combination of brightness, monochromaticity, and high-reflectivity optics availability. Attempts at improving laser performance using proximate feedback optics failed. Modest success has been found to date in ''double foil'' experiments, involving two x-ray lasers spatially separated by 29 cm and shot sequentially in an ''oscillator-amplifier'' configuration

  8. Collisional redistribution effects on x-ray laser saturation behavior

    International Nuclear Information System (INIS)

    Koch, J.A.; MacGowan, B.J.; Da Silva, L.B.; Matthews, D.J.; Lee, R.W.; London, R.A.; Mrowka, S.; Underwood, J.H.; Batson, P.J.

    1994-06-01

    We recently published a detailed summary of our experimental and theoretical research on Ne-like Se x-ray laser line widths, and one of our conclusions was that collisional redistribution rates are likely to have an effect on the saturation behavior of the 206.4 angstrom Se x-ray laser. In this paper we focus on the effects of collisional redistribution on x-ray laser gain coefficients, and discuss ways of including these effects in existing laser line- transfer models

  9. Laser plasma X-ray for non-destructive inspection

    International Nuclear Information System (INIS)

    Yagi, T.; Kusama, H.

    1995-01-01

    External electric field is applied to the laser produced plasma, and its found that plasma shape in soft X-ray region is changed due to the penetrating electric field. The plasma emits strong hard X-ray, which can be used as a compact light source for non-destructive inspection. (author)

  10. Soft x-ray source by laser produced Xe plasma

    International Nuclear Information System (INIS)

    Amano, Sho; Masuda, Kazuya; Miyamoto, Shuji; Mochizuki, Takayasu

    2010-01-01

    The laser plasma soft X-ray source in the wavelength rage of 5-17 nm was developed, which consisted of the rotating drum system supplying cryogenic Xe target and the high repetition rate pulse Nd:YAG slab laser. We found the maximum conversion efficiency of 30% and it demonstrated the soft X-ray generation with the high repetition rate pulse of 320 pps and the high average power of 20 W. The soft X-ray cylindrical mirror was developed and successfully focused the soft X-ray with an energy intensity of 1.3 mJ/cm 2 . We also succeeded in the plasma debris mitigation with Ar gas. This will allow a long lifetime of the mirror and a focusing power intensity of 400 mW/cm 2 with 320 pps. The high power soft X-ray is useful for various applications. (author)

  11. Fourier-limited seeded soft x-ray laser pulse

    Czech Academy of Sciences Publication Activity Database

    Guilbaud, O.; Tissandier, F.; Goddet, J-P.; Ribière, M.; Sebban, S.; Gautier, J.; Joyeux, D.; Ros, D.; Cassou, K.; Kazamias, S.; Klisnick, A.; Habib, J.; Zeitoun, P.; Benredjem, D.; Mocek, Tomáš; Nejdl, Jaroslav; De Rossi, S.; Maynard, G.; Cros, B.; Boudaa, A.; Calisti, A.

    2010-01-01

    Roč. 35, č. 9 (2010), s. 1326-1328 ISSN 0146-9592 Grant - others:AVČR(CZ) M100100911 Institutional research plan: CEZ:AV0Z10100523 Keywords : lasers and laser optics * UV * EUV * x-ray lasers * spectroscopy Subject RIV: BH - Optics, Masers, Lasers Impact factor: 3.316, year: 2010

  12. Review of soft x-ray lasers and their applications

    International Nuclear Information System (INIS)

    Skinner, C.H.

    1991-03-01

    The emerging technology of soft x-ray lasers is in a transition phase between the first laboratory demonstrations of gain and the acceptance of soft x-ray lasers as practical tools for novel applications. Current research is focused on several fronts. The operational wavelength range has been extended to the ''water window'', important for applications in the life sciences. Gain has also been generated with substantially simpler technology (such as a 6J laser) and this augurs well for the commercially availability in the near future of soft x-ray lasers for a variety of applications. Advanced soft x-ray laser concepts are being developed from investigations into ultra-high intensity laser/matter interactions. The first paper a brief historical perspective of x-ray microscopy and holography have begun. In this paper a brief historical perspective of x-ray laser development will be followed by a review of recent advances in recombination, collisional and photo-pumped systems and applications. A summary of current gain-length performance achieved in laboratories worldwide is presented. Near term prospects for applications to novel fields are discussed. 81 refs., 9 figs., 1 tab

  13. X-ray laser interferometry: A new tool for AGEX

    International Nuclear Information System (INIS)

    Wan, A.S.; Moreno, J.C.; Libby, S.B.

    1995-10-01

    Collisionally pumped soft x-ray lasers now operate over a wavelength range extending from 4--40 nm. With the recent advances in the development of multilayer mirrors and beamsplitters in the soft x-ray regime, we can utilize the unique properties of x-ray lasers to study large, rapidly evolving laser-driven plasmas with high electron densities. By employing a shorter wavelength x-ray laser, as compared to using conventional optical laser as the probe source, we can access a much higher density regime while reducing refractive effects which limit the spatial resolution and data interpretation. Using a neon-like yttrium x-ray laser which operates at a wavelength of 15.5 mn, we have performed a series of soft x-ray laser interferometry experiments, operated in the skewed Mach-Zehnder configuration, to characterize plasmas relevant to both weapons and inertial confinement fusion. The two-dimensional density profiles obtained from the interferograms allow us to validate and benchmark our numerical models used to study the physics in the high-energy density regime, relevant to both weapons and inertial confinement fusion

  14. Ultrafast laser pump/x-ray probe experiments

    International Nuclear Information System (INIS)

    Larsson, J.; Judd, E.; Schuck, P.J.

    1997-01-01

    In an ongoing project aimed at probing solids using x-rays obtained at the ALS synchrotron with a sub-picosecond time resolution following interactions with a 100 fs laser pulse, the authors have successfully performed pump-probe experiments limited by the temporal duration of ALS-pulse. They observe a drop in the diffraction efficiency following laser heating. They can attribute this to a disordering of the crystal. Studies with higher temporal resolution are required to determine the mechanism. The authors have also incorporated a low-jitter streakcamera as a diagnostic for observing time-dependant x-ray diffraction. The streakcamera triggered by a photoconductive switch was operated at kHz repetition rates. Using UV-pulses, the authors obtain a temporal response of 2 ps when averaging 5000 laser pulses. They demonstrate the ability to detect monochromatized x-ray radiation from a bend-magnet with the streak camera by measuring the pulse duration of a x-ray pulse to 70 ps. In conclusion, the authors show a rapid disordering of an InSb crystal. The resolution was determined by the duration of the ALS pulse. They also demonstrate that they can detect x-ray radiation from a synchrotron source with a temporal resolution of 2ps, by using an ultrafast x-ray streak camera. Their set-up will allow them to pursue laser pump/x-ray probe experiments to monitor structural changes in materials with ultrafast time resolution

  15. Contact microscopy with a soft x-ray laser

    International Nuclear Information System (INIS)

    DiCicco, D.S.; Kim, D.; Rosser, R.J.; Skinner, C.H.; Suckewer, S.; Gupta, A.P.; Hirschberg, J.G.

    1989-03-01

    A soft x-ray laser of output energy 1-3 mJ at 19.2 nm has been used to record high resolution images of biological specimens. The contact images were recorded on photoresist which was later viewed in a scanning electron microscope. We also present a Composite Optical X- ray Laser Microscope ''COXRALM'' of novel design. 14 refs., 8 figs., 1 tab

  16. Developments in time-resolved x-ray research at APS beamline 7ID

    Energy Technology Data Exchange (ETDEWEB)

    Walko, D. A., E-mail: d-walko@anl.gov; Adams, B. W.; Doumy, G.; Dufresne, E. M.; Li, Yuelin; March, A. M.; Sandy, A. R.; Wang, Jin; Wen, Haidan; Zhu, Yi [Advanced Photon Source, Argonne National Laboratory, Argonne, IL 60439 (United States)

    2016-07-27

    The 7ID beamline of the Advanced Photon Source (APS) is dedicated to time-resolved research using x-ray imaging, scattering, and spectroscopy techniques. Time resolution is achieved via gated detectors and/or mechanical choppers in conjunction with the time structure of the x-ray beam. Three experimental hutches allow for a wide variety of experimental setups. Major areas of research include atomic, molecular, and optical physics; chemistry; condensed matter physics in the bulk, thin film, and surface regimes; and fluid-spray dynamics. Recent developments in facilities at 7ID include a high-power, high-repetition-rate picosecond laser to complement the 1 kHz ultrafast laser. For the ultrafast laser, a newly commissioned optical parametric amplifier provides pump wavelength from 0.2 to 15 µm with energy per pulse up to 200 µJ. A nanodiffraction station has also been commissioned, using Fresnel zone-plate optics to achieve a focused x-ray spot of 300 nm. This nanoprobe is not only used to spatially resolve the evolution of small features in samples after optical excitation, but also has been combined with an intense THz source to study material response under ultrafast electric fields.

  17. Spectral and imaging characterization of tabletop X-ray lasers

    Energy Technology Data Exchange (ETDEWEB)

    Dunn, J.; Osterheld, A.L.; Moon, S.J.; Fournier, K.B.; Nilsen, J. [Lawrence Livermore National Lab., CA (United States); Faenov, A.Ya.; Pikuz, T.A.; Skobelev, I.Yu.; Magunov, A.I. [Lawrence Livermore National Lab., CA (United States); MISDC of VNIIFTRI, Mendeleevo (Russian Federation); Shlyaptsev, V.N. [Lawrence Livermore National Lab., CA (United States); California Univ., Davis, CA (United States). DAS

    2001-07-01

    We have performed L-shell spectroscopy and one-dimensional (1-D) imaging of a line focus plasma from a laser-heated Fe polished slab using the tabletop COMET laser system at the Lawrence Livermore National Laboratory. These plasmas are used to generate a Ne-like Fe transient gain X-ray laser that is recorded simultaneously. A spherically-curved crystal spectrometer gives high resolution X-ray spectra of the n=3-2 and n=4-2 resonance lines with 1-D spatial resolution along the line focus. Spectra are presented for different laser pulse conditions. In addition, a variety of X-ray imaging techniques are described. We discuss imaging results from a double-slit X-ray camera with a spherically-curved crystal spectrometer. We show a high resolution Fe K-{alpha} spectrum from the X-ray laser target that indicates the presence of hot electrons in the X-ray laser plasma. (orig.)

  18. Femtosecond X-ray magnetic circular dichroism absorption spectroscopy at an X-ray free electron laser

    Energy Technology Data Exchange (ETDEWEB)

    Higley, Daniel J., E-mail: dhigley@stanford.edu; Yuan, Edwin [SLAC National Accelerator Laboratory, 2575 Sand Hill Road, Menlo Park, California 94025 (United States); Department of Applied Physics, Stanford University, Stanford, California 94305 (United States); Hirsch, Konstantin; Dakovski, Georgi L.; Jal, Emmanuelle; Lutman, Alberto A.; Coslovich, Giacomo; Hart, Philip; Hoffmann, Matthias C.; Mitra, Ankush; Moeller, Stefan; Ohldag, Hendrik; Seaberg, Matthew; Stöhr, Joachim; Nuhn, Heinz-Dieter; Reid, Alex H.; Dürr, Hermann A.; Schlotter, William F. [SLAC National Accelerator Laboratory, 2575 Sand Hill Road, Menlo Park, California 94025 (United States); Liu, Tianmin; MacArthur, James P. [SLAC National Accelerator Laboratory, 2575 Sand Hill Road, Menlo Park, California 94025 (United States); Department of Physics, Stanford University, Stanford, California 94305 (United States); and others

    2016-03-15

    X-ray magnetic circular dichroism spectroscopy using an X-ray free electron laser is demonstrated with spectra over the Fe L{sub 3,2}-edges. The high brightness of the X-ray free electron laser combined with high accuracy detection of incident and transmitted X-rays enables ultrafast X-ray magnetic circular dichroism studies of unprecedented sensitivity. This new capability is applied to a study of all-optical magnetic switching dynamics of Fe and Gd magnetic sublattices in a GdFeCo thin film above its magnetization compensation temperature.

  19. High-intensity laser synchrotron x-ray source

    International Nuclear Information System (INIS)

    Pogorelsky, I.V.

    1995-10-01

    A laser interacting with a relativistic electron beam behaves like a virtual wiggler of an extremely short period equal to half of the laser wavelength. This approach opens a route to relatively compact, high-brightness x-ray sources alternative or complementary to conventional synchrotron light sources. Although not new, the Laser Synchrotron Light Source (LSLS) concept is still waiting for a convincing demonstration. Available at the BNL's Accelerator Test Facility (ATF), a high-brightness electron beam and the high-power C0 2 laser may be used as prototype LSLS brick stones. In a feasible demonstration experiment, 10-GW, 100-ps C0 2 laser beam will be brought to a head-on collision with a 10-ps, 0.5-nC, 70 MeV electron bunch. Flashes of well-collimated, up to 9.36-keV (∼ Angstrom) x-rays of 10-ps pulse duration, with a flux of ∼10 19 photons/sec will be produced via linear Compton backscattering. The x-ray spectrum is tunable proportionally to a variable e-beam energy. A natural short-term extension of the proposed experiment would be further enhancement of the x-ray flux to a 10 21 -10 22 photons/sec level, after the ongoing ATF CO 2 laser upgrade to 1 TW peak power and electron bunch shortening to 3 ps. The ATF LSLS x-ray beamline, exceeding by orders of magnitude the peak fluxes attained at the National Synchrotron Light Source (NSLS) x-ray storage ring, may become attractive for certain users, e.g., for biological x-ray microscopy. In addition, a terawatt CO 2 laser will enable harmonic multiplication of the x-ray spectrum via nonlinear Compton scattering

  20. Characterization of X-ray emission from laser generated plasma

    Science.gov (United States)

    Cannavò, Antonino; Torrisi, Lorenzo; Ceccio, Giovanni; Cutroneo, Mariapompea; Calcagno, Lucia; Sciuto, Antonella; Mazzillo, Massimo

    2018-01-01

    X-ray emission from laser generated plasma was studied at low (1010 W/cm2) and high (1018 W/cm2) intensity using ns and fs laser, respectively. Plasma characteristics were controlled trough the laser parameters, the irradiation conditions and the target properties. The X-ray spectra were acquired using fast detection technique based on SiC diodes with different active regions. The X-ray yield increases with the atomic number of the target, both at low and high intensity, and a similar empirical law has been obtained. The X-ray emission mechanisms from plasma are correlated to the plasma temperature and density and to the Coulomb charge particle acceleration, due to the charge separation effects produced in the non-equilibrium plasma. Functional dependences, theoretical approaches and interpretation of possible mechanism will be presented and discussed.

  1. Characterization of X-ray emission from laser generated plasma

    Directory of Open Access Journals (Sweden)

    Cannavò Antonino

    2018-01-01

    Full Text Available X-ray emission from laser generated plasma was studied at low (1010 W/cm2 and high (1018 W/cm2 intensity using ns and fs laser, respectively. Plasma characteristics were controlled trough the laser parameters, the irradiation conditions and the target properties. The X-ray spectra were acquired using fast detection technique based on SiC diodes with different active regions. The X-ray yield increases with the atomic number of the target, both at low and high intensity, and a similar empirical law has been obtained. The X-ray emission mechanisms from plasma are correlated to the plasma temperature and density and to the Coulomb charge particle acceleration, due to the charge separation effects produced in the non-equilibrium plasma. Functional dependences, theoretical approaches and interpretation of possible mechanism will be presented and discussed.

  2. 13th International Conference on X-Ray Lasers

    CERN Document Server

    Gautier, Julien; Ros, David; Zeitoun, Philippe

    2014-01-01

    These proceedings comprise of invited and contributed papers presented at the 13th International Conference on X-Ray Lasers (ICXRL 2012) which was held 11–15 June 2012 in Paris, in the famous Quartier Latin, inside the historical Center of Cordeliers. This conference is part of a continuing series dedicated to recent developments and applications of x-ray lasers and other coherent x-ray sources with attention to supporting technologies and instrumentation. New results in the generation of intense, coherent x-rays and progress towards practical devices and their applications are reported in these proceedings, including areas of research in plasma-based x-ray lasers, 4th generation accelerator-based sources and higher harmonic generation. Recent achievements related to the increase of the repetition rate up to 100 Hz and shorter wavelength collisional plasma-based soft x-ray lasers down to about 7 nm are presented. Seeding the amplifying plasma with a femtosecond high-order harmonic of infrared laser was fore...

  3. Time-resolved X-ray PIV technique for diagnosing opaque biofluid flow with insufficient X-ray fluxes.

    Science.gov (United States)

    Jung, Sung Yong; Park, Han Wook; Kim, Bo Heum; Lee, Sang Joon

    2013-05-01

    X-ray imaging is used to visualize the biofluid flow phenomena in a nondestructive manner. A technique currently used for quantitative visualization is X-ray particle image velocimetry (PIV). Although this technique provides a high spatial resolution (less than 10 µm), significant hemodynamic parameters are difficult to obtain under actual physiological conditions because of the limited temporal resolution of the technique, which in turn is due to the relatively long exposure time (~10 ms) involved in X-ray imaging. This study combines an image intensifier with a high-speed camera to reduce exposure time, thereby improving temporal resolution. The image intensifier amplifies light flux by emitting secondary electrons in the micro-channel plate. The increased incident light flux greatly reduces the exposure time (below 200 µs). The proposed X-ray PIV system was applied to high-speed blood flows in a tube, and the velocity field information was successfully obtained. The time-resolved X-ray PIV system can be employed to investigate blood flows at beamlines with insufficient X-ray fluxes under specific physiological conditions. This method facilitates understanding of the basic hemodynamic characteristics and pathological mechanism of cardiovascular diseases.

  4. Soft x-ray laser experiments at Novette Laser Facility

    International Nuclear Information System (INIS)

    Matthews, D.; Hagelstein, P.; Rosen, M.

    1984-01-01

    We discuss the results of and future plans for experiments to study the possibility of producing an x-ray laser. The schemes we have investigated are all pumped by the Novette Laser, operated at short pulse (tau/sub L/ approx. 100 psec) and an incident wavelength of lambda /sub L/ approx. 0.53 μm. We have studied the possibility of lasing at 53.6, 68.0 to 72.0, 119.0, and 153.0 eV, using the inversion methods of resonant photo-excitation, collisional excitation, and three-body recombination

  5. Guest–Host Interactions Investigated by Time-Resolved X-ray Spectroscopies and Scattering at MHz Rates

    DEFF Research Database (Denmark)

    Haldrup, Martin Kristoffer; Vanko, G.; Gawelda, W.

    2012-01-01

    We have studied the photoinduced low spin (LS) to high spin (HS) conversion of [Fe(bipy)3]2+ in aqueous solution. In a laser pump/X-ray probe synchrotron setup permitting simultaneous, time-resolved X-ray diffuse scattering (XDS) and X-ray spectroscopic measurements at a 3.26 MHz repetition rate...... lifetime, allowing the detection of an ultrafast change in bulk solvent density. An analysis approach directly utilizing the spectroscopic data in the XDS analysis effectively reduces the number of free parameters, and both combined permit extraction of information about the ultrafast structural dynamics...

  6. X-ray laser related experiments and theory at Princeton

    International Nuclear Information System (INIS)

    Suckewer, S.

    1989-04-01

    This paper describes a new system for the development of an x-ray laser in the wavelength region from 5 nm to 1 nm utilizing a Powerful Sub-Picosecond Laser (PP-Laser) of expected peak power up to 0.5 TW in a 300 fs pulse. Soft x-ray spectra generated by the interaction of the PP-Laser beam with different targets are presented and compared to the spectra generated by a much less intense laser beam (20--30 GW). A theoretical model for the interaction of atoms with such a strong laser EM field is also briefly discussed. The development of additional amplifiers for the recombining soft x-ray laser and the design of a cavity are presented from the point of view of applications for x-ray microscopy and microlithography. This overview concludes with the presentation of recent results on the quenching of spontaneous emission radiation and its possible effect on the absolute intensity calibration of soft x-ray spectrometers. 26 refs., 18 figs

  7. X-ray generation by femtosecond laser pulses and its application to soft X-ray imaging microscope

    International Nuclear Information System (INIS)

    Ikeda, Kenichi; Kotaki, Hideyuki; Nakajima, Kazuhisa

    2002-01-01

    We have developed laser-produced plasma X-ray sources using femtosecond laser pulses at 10Hz repetition rate in a table-top size in order to investigate basic mechanism of X-ray emission from laser-matter interactions and its application to a X-ray microscope. In a soft X-ray region over 5 nm wavelength, laser-plasma X-ray emission from a solid target achieved an intense flux of photons of the order of 1011 photons/rad per pulse with duration of a few 100 ps, which is intense enough to make a clear imaging in a short time exposure. As an application of laser-produced plasma X-ray source, we have developed a soft X-ray imaging microscope operating in the wavelength range around 14 nm. The microscope consists of a cylindrically ellipsoidal condenser mirror and a Schwarzshird objective mirror with highly-reflective multilayers. We report preliminary results of performance tests of the soft X-ray imaging microscope with a compact laser-produced plasma X-ray source

  8. 11th International Conference on X-Ray Lasers

    CERN Document Server

    Lewis, Ciaran L. S; X-Ray Lasers 2008

    2009-01-01

    This book provides a thorough account of the current status of achievements made in the area of soft X-ray laser source development and of the increasingly diverse applications being demonstrated using such radiation sources. There is significant effort worldwide to develop very bright, short duration radiation sources in the X-ray spectral region – driven by the multitude of potential applications in all branches of science. This book contains updates on several different approaches for comparative purposes but concentrates on developments in the area of laser-produced plasmas, whereby transient population inversion and gain between ion states is pumped by optical lasers interacting with pre-formed plasmas. The most significant development here is the demonstrated increasing feasibility to produce useful soft X-ray laser beams with high repetition rates in a typical, small, university-class laboratory – as opposed to the requirement of access to a national facility some 20 years ago. Experimental progres...

  9. P 8: Table-top instrumentation for time-resolved luminescence spectroscopy of solids excited by soft X-ray from a laser induced plasma source and/or UV-VIS laser

    International Nuclear Information System (INIS)

    Bruza, P.; Fidler, V.; Nikl, M.

    2010-01-01

    The design and use of a novel, table-top UV-VIS luminescence spectrometer with two excitation sources is described: a soft X-ray/XUV pulse excitation from the laser-produced plasma in gas puff target of about 4 ns duration, and a conventional N 2 pulse laser excitation at 337 nm (or any other UV-VIS pulse laser excitation). The XUV plasma source generates photons of either quasi-monochromatic (N target, E = 430 eV) or wide (Ar target, E = 200 ∼ 600 eV) spectral range. A combination of both X-ray/XUV and UV-VIS excitation in one experimental apparatus allows to perform comparative luminescence spectra and kinetics measurements under the same experimental conditions. In order to demonstrate the spectrometer, the UV-VIS luminescence spectra and decay kinetics of cerium doped Lu 3 Al 5 O 12 single crystal (LuAG:Ce) scintillator excited by XUV and UV radiation were acquired. Luminescence of doped Ce 3+ ions was studied under XUV 430 eV excitation from the laser-produced nitrogen plasma, and compared with the luminescence under 337 nm (3,68 eV) UV excitation from nitrogen laser. In the former case the excitation energy is deposited in the LuAG host, while in the latter the 4f-5d transition of Ce 3+ is directly excited. Furthermore, LuAG:Ce single crystals and single crystalline films luminescence decay profiles are compared and discussed. (authors)

  10. Watching proteins function with time-resolved x-ray crystallography

    International Nuclear Information System (INIS)

    Šrajer, Vukica; Schmidt, Marius

    2017-01-01

    Macromolecular crystallography was immensely successful in the last two decades. To a large degree this success resulted from use of powerful third generation synchrotron x-ray sources. An expansive database of more than 100 000 protein structures, of which many were determined at resolution better than 2 Å, is available today. With this achievement, the spotlight in structural biology is shifting from determination of static structures to elucidating dynamic aspects of protein function. A powerful tool for addressing these aspects is time-resolved crystallography, where a genuine biological function is triggered in the crystal with a goal of capturing molecules in action and determining protein kinetics and structures of intermediates (Schmidt et al 2005a Methods Mol. Biol . 305 115–54, Schmidt 2008 Ultrashort Laser Pulses in Biology and Medicine (Berlin: Springer) pp 201–41, Neutze and Moffat 2012 Curr. Opin. Struct. Biol . 22 651–9, Šrajer 2014 The Future of Dynamic Structural Science (Berlin: Springer) pp 237–51). In this approach, short and intense x-ray pulses are used to probe intermediates in real time and at room temperature, in an ongoing reaction that is initiated synchronously and rapidly in the crystal. Time-resolved macromolecular crystallography with 100 ps time resolution at synchrotron x-ray sources is in its mature phase today, particularly for studies of reversible, light-initiated reactions. The advent of the new free electron lasers for hard x-rays (XFELs; 5–20 keV), which provide exceptionally intense, femtosecond x-ray pulses, marks a new frontier for time-resolved crystallography. The exploration of ultra-fast events becomes possible in high-resolution structural detail, on sub-picosecond time scales (Tenboer et al 2014 Science 346 1242–6, Barends et al 2015 Science 350 445–50, Pande et al 2016 Science 352 725–9). We review here state-of-the-art time-resolved crystallographic experiments both at synchrotrons and XFELs

  11. Watching proteins function with time-resolved x-ray crystallography

    Science.gov (United States)

    Šrajer, Vukica; Schmidt, Marius

    2017-09-01

    Macromolecular crystallography was immensely successful in the last two decades. To a large degree this success resulted from use of powerful third generation synchrotron x-ray sources. An expansive database of more than 100 000 protein structures, of which many were determined at resolution better than 2 Å, is available today. With this achievement, the spotlight in structural biology is shifting from determination of static structures to elucidating dynamic aspects of protein function. A powerful tool for addressing these aspects is time-resolved crystallography, where a genuine biological function is triggered in the crystal with a goal of capturing molecules in action and determining protein kinetics and structures of intermediates (Schmidt et al 2005a Methods Mol. Biol. 305 115-54, Schmidt 2008 Ultrashort Laser Pulses in Biology and Medicine (Berlin: Springer) pp 201-41, Neutze and Moffat 2012 Curr. Opin. Struct. Biol. 22 651-9, Šrajer 2014 The Future of Dynamic Structural Science (Berlin: Springer) pp 237-51). In this approach, short and intense x-ray pulses are used to probe intermediates in real time and at room temperature, in an ongoing reaction that is initiated synchronously and rapidly in the crystal. Time-resolved macromolecular crystallography with 100 ps time resolution at synchrotron x-ray sources is in its mature phase today, particularly for studies of reversible, light-initiated reactions. The advent of the new free electron lasers for hard x-rays (XFELs; 5-20 keV), which provide exceptionally intense, femtosecond x-ray pulses, marks a new frontier for time-resolved crystallography. The exploration of ultra-fast events becomes possible in high-resolution structural detail, on sub-picosecond time scales (Tenboer et al 2014 Science 346 1242-6, Barends et al 2015 Science 350 445-50, Pande et al 2016 Science 352 725-9). We review here state-of-the-art time-resolved crystallographic experiments both at synchrotrons and XFELs. We also outline

  12. Watching proteins function with time-resolved x-ray crystallography

    Energy Technology Data Exchange (ETDEWEB)

    Šrajer, Vukica; Schmidt, Marius

    2017-08-22

    Macromolecular crystallography was immensely successful in the last two decades. To a large degree this success resulted from use of powerful third generation synchrotron x-ray sources. An expansive database of more than 100 000 protein structures, of which many were determined at resolution better than 2 Å, is available today. With this achievement, the spotlight in structural biology is shifting from determination of static structures to elucidating dynamic aspects of protein function. A powerful tool for addressing these aspects is time-resolved crystallography, where a genuine biological function is triggered in the crystal with a goal of capturing molecules in action and determining protein kinetics and structures of intermediates (Schmidt et al 2005a Methods Mol. Biol. 305 115–54, Schmidt 2008 Ultrashort Laser Pulses in Biology and Medicine (Berlin: Springer) pp 201–41, Neutze and Moffat 2012 Curr. Opin. Struct. Biol. 22 651–9, Šrajer 2014 The Future of Dynamic Structural Science (Berlin: Springer) pp 237–51). In this approach, short and intense x-ray pulses are used to probe intermediates in real time and at room temperature, in an ongoing reaction that is initiated synchronously and rapidly in the crystal. Time-resolved macromolecular crystallography with 100 ps time resolution at synchrotron x-ray sources is in its mature phase today, particularly for studies of reversible, light-initiated reactions. The advent of the new free electron lasers for hard x-rays (XFELs; 5–20 keV), which provide exceptionally intense, femtosecond x-ray pulses, marks a new frontier for time-resolved crystallography. The exploration of ultra-fast events becomes possible in high-resolution structural detail, on sub-picosecond time scales (Tenboer et al 2014 Science 346 1242–6, Barends et al 2015 Science 350 445–50, Pande et al 2016 Science 352 725–9). We review here state-of-the-art time-resolved crystallographic experiments both at synchrotrons and XFELs. We

  13. Temporal characteristic analysis of laser-modulated pulsed X-ray source for space X-ray communication

    Science.gov (United States)

    Hang, Shuang; Liu, Yunpeng; Li, Huan; Tang, Xiaobin; Chen, Da

    2018-04-01

    X-ray communication (XCOM) is a new communication type and is expected to realize high-speed data transmission in some special communication scenarios, such as deep space communication and blackout communication. This study proposes a high-speed modulated X-ray source scheme based on the laser-to-X-ray conversion. The temporal characteristics of the essential components of the proposed laser-modulated pulsed X-ray source (LMPXS) were analyzed to evaluate its pulse emission performance. Results show that the LMPXS can provide a maximum modulation rate up to 100 Mbps which is expected to significantly improve the data rate of XCOM.

  14. Techniques for synchronization of X-Ray pulses to the pump laser in an ultrafast X-Ray facility

    International Nuclear Information System (INIS)

    Corlett, J.N.; Doolittle, L.; Schoenlein, R.; Staples, J.; Wilcox, R.; Zholents, A.

    2003-01-01

    Accurate timing of ultrafast x-ray probe pulses emitted from a synchrotron radiation source with respect to the signal initiating a process in the sample under study is critical for the investigation of structural dynamics in the femtosecond regime. We describe schemes for achieving accurate timing of femtosecond x-ray synchrotron radiation pulses relative to a pump laser, where x-rays pulses of <100 fs duration are generated from the proposed LUX source based on a recirculating superconducting linac. We present a description of the timing signal generation and distribution systems to minimize timing jitter of the x-rays relative to the experimental lasers

  15. Soft x-ray streak camera for laser fusion applications

    International Nuclear Information System (INIS)

    Stradling, G.L.

    1981-04-01

    This thesis reviews the development and significance of the soft x-ray streak camera (SXRSC) in the context of inertial confinement fusion energy development. A brief introduction of laser fusion and laser fusion diagnostics is presented. The need for a soft x-ray streak camera as a laser fusion diagnostic is shown. Basic x-ray streak camera characteristics, design, and operation are reviewed. The SXRSC design criteria, the requirement for a subkilovolt x-ray transmitting window, and the resulting camera design are explained. Theory and design of reflector-filter pair combinations for three subkilovolt channels centered at 220 eV, 460 eV, and 620 eV are also presented. Calibration experiments are explained and data showing a dynamic range of 1000 and a sweep speed of 134 psec/mm are presented. Sensitivity modifications to the soft x-ray streak camera for a high-power target shot are described. A preliminary investigation, using a stepped cathode, of the thickness dependence of the gold photocathode response is discussed. Data from a typical Argus laser gold-disk target experiment are shown

  16. 10th International Conference on X-Ray Lasers

    CERN Document Server

    Nickles, P.V; X-Ray Lasers 2006

    2007-01-01

    The search for table-top and repetitive pump schemes during the last decade has been the driving force behind the spectacular advances demonstrated during the 10th International Conference on X-Ray Lasers, organized in 2006 in Berlin. Since 1986, international experts have gathered every two years at this established conference to discuss the progress in theory, experiment and application of plasma-based soft X-ray lasers. Traditionally, the conference sessions devoted to complementary and alternative sources of short wavelength radiation, such as high harmonics, XFEL or incoherent X-rays are organized so as to emphasize the role of X-ray laser research in relation to the other short wavelength sources. Grazing incidence pumping (GRIP) and seeding with high harmonics were the dominant topics of the conference. High repetition rate and portable X-ray lasers were reported to have been applied in metrology and photochemistry for the first time. The proceedings of this series of conferences constitute a comprehen...

  17. Theory and analysis of soft x-ray laser experiments

    International Nuclear Information System (INIS)

    Whitten, B.L.; Hazi, A.U.

    1985-10-01

    The atomic modeling of soft x-ray laser schemes presents a formidable challenge to the theorists - a challenge magnified by the recent successful experiments. A complex plasma environment with many ion species present must be simulated. Effects such as turbulence, time dependence, and radiation transport, which are very difficult to model accurately, may be important. We shall describe our efforts to model the recently demonstrated soft x-ray laser in collisionally pumped neon-like selenium, with emphasis on the ionization balance and excited state kinetics. The relative importance of various atomic processes, such as collisional excitation and dielectronic recombination, on the inversion kinetics will be demonstrated. We shall compare our models with experimental results and evaluate the success of this technique in predicting and analyzing the results of x-ray laser experiments. 22 refs., 5 figs., 3 tabs

  18. Time-resolved soft x-ray absorption setup using multi-bunch operation modes at synchrotrons

    International Nuclear Information System (INIS)

    Stebel, L.; Sigalotti, P.; Ressel, B.; Cautero, G.; Malvestuto, M.; Capogrosso, V.; Bondino, F.; Magnano, E.; Parmigiani, F.

    2011-01-01

    Here, we report on a novel experimental apparatus for performing time-resolved soft x-ray absorption spectroscopy in the sub-ns time scale using non-hybrid multi-bunch mode synchrotron radiation. The present setup is based on a variable repetition rate Ti:sapphire laser (pump pulse) synchronized with the ∼500 MHz x-ray synchrotron radiation bunches and on a detection system that discriminates and singles out the significant x-ray photon pulses by means of a custom made photon counting unit. The whole setup has been validated by measuring the time evolution of the L 3 absorption edge during the melting and the solidification of a Ge single crystal irradiated by an intense ultrafast laser pulse. These results pave the way for performing synchrotron time-resolved experiments in the sub-ns time domain with variable repetition rate exploiting the full flux of the synchrotron radiation.

  19. Flash X-Ray (FXR) Accelerator Optimization Electronic Time-Resolved Measurement of X-Ray Source Size

    International Nuclear Information System (INIS)

    Jacob, J; Ong, M; Wargo, P

    2005-01-01

    Lawrence Livermore National Laboratory (LLNL) is currently investigating various approaches to minimize the x-ray source size on the Flash X-Ray (FXR) linear induction accelerator in order to improve x-ray flux and increase resolution for hydrodynamic radiography experiments. In order to effectively gauge improvements to final x-ray source size, a fast, robust, and accurate system for measuring the spot size is required. Timely feedback on x-ray source size allows new and improved accelerator tunes to be deployed and optimized within the limited run-time constraints of a production facility with a busy experimental schedule; in addition, time-resolved measurement capability allows the investigation of not only the time-averaged source size, but also the evolution of the source size, centroid position, and x-ray dose throughout the 70 ns beam pulse. Combined with time-resolved measurements of electron beam parameters such as emittance, energy, and current, key limiting factors can be identified, modeled, and optimized for the best possible spot size. Roll-bar techniques are a widely used method for x-ray source size measurement, and have been the method of choice at FXR for many years. A thick bar of tungsten or other dense metal with a sharp edge is inserted into the path of the x-ray beam so as to heavily attenuate the lower half of the beam, resulting in a half-light, half-dark image as seen downstream of the roll-bar; by measuring the width of the transition from light to dark across the edge of the roll-bar, the source size can be deduced. For many years, film has been the imaging medium of choice for roll-bar measurements thanks to its high resolution, linear response, and excellent contrast ratio. Film measurements, however, are fairly cumbersome and require considerable setup and analysis time; moreover, with the continuing trend towards all-electronic measurement systems, film is becoming increasingly difficult and expensive to procure. Here, we shall

  20. Bright ultrashort x-rays from intense subpicosecond laser-plasma interactions

    International Nuclear Information System (INIS)

    Umstadter, D.

    1995-01-01

    Short-pulse, high-intensity lasers interacting with solid targets make possible the study of a new class of laser-plasma interactions. They are unique because during the ultrashort laser pulse relatively little expansion occurs, and the density scale length remains much less than the laser wavelength. This makes possible the direct deposition of a significant amount of the laser energy at close to solid density. Steep plasma temperature and density gradients subsequently cause rapid cooling, resulting in highly non-equilibrium conditions and the concurrent emission of extremely bright ultrashort x-ray pulses. In this study, the latter are investigated experimentally with temporally and spectrally resolved soft x-ray diagnostics. The emitted x-ray spectra from solid targets with various atomic numbers are characterized for a laser pulse width τ l ∼ 400 fs. These ultrashort x rays may be used as (1) a diagnostic of solid-density plasma conditions, (2) a tool for the study of radiation hydrodynamics in a parameter regime that is otherwise inaccessible, and (3) a source for time-resolved diffraction, spectroscopy, or microscopy studies of transient chemical, biological or physical phenomena

  1. A synchrotron radiation camera and data acquisition system for time resolved x-ray scattering studies

    International Nuclear Information System (INIS)

    Bordas, J.; Koch, M.H.J.; Clout, P.N.; Dorrington, E.; Boulin, C.; Gabriel, A.

    1980-01-01

    Until recently, time resolved measurements of x-ray scattering patterns have not been feasible because laboratory x-ray sources were too weak and detectors unavailable. Recent developments in both these fields have changed the situation, and it is now possible to follow changes in x-ray scattering patterns with a time resolution of a few ms. The apparatus used to achieve this is described and some examples from recent biological experiments are given. (author)

  2. X-ray imaging in the laser-fusion program

    International Nuclear Information System (INIS)

    McCall, G.H.

    1977-01-01

    Imaging devices which are used or planned for x-ray imaging in the laser-fusion program are discussed. Resolution criteria are explained, and a suggestion is made for using the modulation transfer function as a uniform definition of resolution for these devices

  3. Experiments on resonantly photo-pumped x-ray lasers

    International Nuclear Information System (INIS)

    Nilsen, J.; Porter, J.L.; Da Silva, L.B.; MacGowan, B.; Beiersdorfer, P..; Elliott, S.R.; Young, B.K.

    1992-01-01

    We describe our recent effort to identify and study a promising resonantly photopumped x-ray laser scheme. In particular we will describe a scheme which uses the strong emission lines of a nickel-like ion to resonantly photo-pump a neon-like ion and enhance the lasing of the neon-like 3p → 3s transitions

  4. The complex ion structure of warm dense carbon measured by spectrally resolved x-ray scattering

    Energy Technology Data Exchange (ETDEWEB)

    Kraus, D.; Barbrel, B.; Falcone, R. W. [Department of Physics, University of California, Berkeley, California 94720 (United States); Vorberger, J. [Max-Planck-Institut für Physik komplexer Systeme, Nöthnitzer Straße 38, 01187 Dresden (Germany); Helfrich, J.; Frydrych, S.; Ortner, A.; Otten, A.; Roth, F.; Schaumann, G.; Schumacher, D.; Siegenthaler, K.; Wagner, F.; Roth, M. [Institut für Kernphysik, Technische Universität Darmstadt, Schlossgartenstraße 9, 64289 Darmstadt (Germany); Gericke, D. O.; Wünsch, K. [Centre for Fusion, Space and Astrophysics, Department of Physics, University of Warwick, Coventry CV4 7AL (United Kingdom); Bachmann, B.; Döppner, T. [Lawrence Livermore National Laboratory, Livermore, California 94550 (United States); Bagnoud, V.; Blažević, A. [GSI Helmholtzzentrum für Schwerionenforschung GmbH, Planckstraße 1, 64291 Darmstadt (Germany); and others

    2015-05-15

    We present measurements of the complex ion structure of warm dense carbon close to the melting line at pressures around 100 GPa. High-pressure samples were created by laser-driven shock compression of graphite and probed by intense laser-generated x-ray sources with photon energies of 4.75 keV and 4.95 keV. High-efficiency crystal spectrometers allow for spectrally resolving the scattered radiation. Comparing the ratio of elastically and inelastically scattered radiation, we find evidence for a complex bonded liquid that is predicted by ab-initio quantum simulations showing the influence of chemical bonds under these conditions. Using graphite samples of different initial densities we demonstrate the capability of spectrally resolved x-ray scattering to monitor the carbon solid-liquid transition at relatively constant pressure of 150 GPa. Showing first single-pulse scattering spectra from cold graphite of unprecedented quality recorded at the Linac Coherent Light Source, we demonstrate the outstanding possibilities for future high-precision measurements at 4th Generation Light Sources.

  5. Time Resolved X-Ray Spot Size Diagnostic

    CERN Document Server

    Richardson, Roger; Falabella, Steven; Guethlein, Gary; Raymond, Brett; Weir, John

    2005-01-01

    A diagnostic was developed for the determination of temporal history of an X-ray spot. A pair of thin (0.5 mm) slits image the x-ray spot to a fast scintillator which is coupled to a fast detector, thus sampling a slice of the X-Ray spot. Two other scintillator/detectors are used to determine the position of the spot and total forward dose. The slit signal is normalized to the dose and the resulting signal is analyzed to get the spot size. The position information is used to compensate for small changes due to spot motion and misalignment. The time resolution of the diagnostic is about 1 ns and measures spots from 0.5 mm to over 3 mm. The theory and equations used to calculate spot size and position are presented, as well as data. The calculations assume a symmetric, Gaussian spot. The spot data is generated by the ETA II accelerator, a 2kA, 5.5 MeV, 60ns electron beam focused on a Tantalum target. The spot generated is typically about 1 mm FWHM. Comparisons are made to an X-ray pinhole camera which images th...

  6. Time-resolved pump-probe X-ray absorption fine structure spectroscopy of Gaq3

    International Nuclear Information System (INIS)

    Dicke, Benjamin

    2013-01-01

    Gallium(tris-8-hydroxyquinoline) (Gaq 3 ) belongs to a class of metal organic compounds, used as electron transport layer and emissive layer in organic light emitting diodes. Many research activities have concentrated on the optical and electronic properties, especially of the homologue molecule aluminum(tris-8-hydroxyquinoline) (Alq 3 ). Knowledge of the first excited state S 1 structure of these molecules could provide deeper insight into the processes involved into the operation of electronic devices, such as OLEDs and, hence, it could further improve their efficiency and optical properties. Until now the excited state structure could not be determined experimentally. Most of the information about this structure mainly arises from theoretical calculations. X-ray absorption fine structure (XAFS) spectroscopy is a well developed technique to determine both, the electronic and the geometric properties of a sample. The connection of ultrashort pulsed X-ray sources with a pulsed laser system offers the possibility to use XAFS as a tool for studying the transient changes of a sample induced by a laser pulse. In the framework of this thesis a new setup for time-resolved pump-probe X-ray absorption spectroscopy at PETRA III beamline P11 was developed for measuring samples in liquid form. In this setup the sample is pumped into its photo-excited state by a femtosecond laser pump pulse with 343 nm wavelength and after a certain time delay probed by an X-ray probe pulse. In this way the first excited singlet state S 1 of Gaq 3 dissolved in benzyl alcohol was analyzed. A structural model for the excited state structure of the Gaq 3 molecule based on the several times reproduced results of the XAFS experiments is proposed. According to this model it was found that the Ga-N A bond length is elongated, while the Ga-O A bond length is shortened upon photoexcitation. The dynamics of the structural changes were not the focus of this thesis. Nevertheless the excited state lifetime

  7. Mode-Locked Multichromatic X-Rays in a Seeded Free-Electron Laser for Single-Shot X-Ray Spectroscopy

    Energy Technology Data Exchange (ETDEWEB)

    Xiang, Dao; Ding, Yuantao; Raubenheimer, Tor; Wu, Juhao; /SLAC

    2012-05-10

    We present the promise of generating gigawatt mode-locked multichromatic x rays in a seeded free-electron laser (FEL). We show that, by using a laser to imprint periodic modulation in electron beam phase space, a single-frequency coherent seed can be amplified and further translated to a mode-locked multichromatic output in an FEL. With this configuration the FEL output consists of a train of mode-locked ultrashort pulses which span a wide frequency gap with a series of equally spaced sharp lines. These gigawatt multichromatic x rays may potentially allow one to explore the structure and dynamics of a large number of atomic states simultaneously. The feasibility of generating mode-locked x rays ranging from carbon K edge ({approx}284 eV) to copper L{sub 3} edge ({approx}931 eV) is confirmed with numerical simulation using the realistic parameters of the linac coherent light source (LCLS) and LCLS-II. We anticipate that the mode-locked multichromatic x rays in FELs may open up new opportunities in x-ray spectroscopy (i.e. resonant inelastic x-ray scattering, time-resolved scattering and spectroscopy, etc.).

  8. Scaling of x-ray emission and ion velocity in laser produced Cu ...

    Indian Academy of Sciences (India)

    Laser plasma; x-ray emission; conversion efficiency; ion velocities. ... fits from this kind of optimization studies are in the fields of x-ray lithography, x-ray lasers etc. .... formula between the x-ray conversion rate versus different parameters of the ...

  9. Excitation mechanisms for XUV and X-ray lasers

    International Nuclear Information System (INIS)

    El-Sherbini, T.M.; Arrubban, M.M.

    1992-01-01

    Two excitation mechanisms leading to lasing action in the extreme ultraviolet and soft X-ray spectral regions are proposed. Boron- like ions of Mg VIII, Al IX and Si X plasmas are used as the active laser material. The upper laser level is the metastable 1s 2 2s 2 4p( 2 p) state while the lower level is the short lived 1s 2 2s 2 3d( 2 D) state. (author). 10 refs, 1 fig., 3 tabs

  10. A Feasibility Experiment for a Soft X-Ray Laser

    Science.gov (United States)

    1976-09-01

    has embarked on a large scale laser fusion program initially aimed at achieving sufficient thermometric yield from a single pellet to initiate a...gold, aluminum ). The report suggests that 10 to 20 percent of the incident laser energy can be converted to X rays below 1 keV. A Lawrence Livermore...Computa- tions of the population inversion for the inner shell electrons, as found in 3 I-.--I~ . . AFWL-TR-76-107 aluminum , indicate a favorable

  11. Progress in the applicability of plasma X-ray lasers

    Energy Technology Data Exchange (ETDEWEB)

    Kuehl, T., E-mail: T.Kuehl@gsi.de; Aurand, B.; Bagnoud, V.; Ecker, B.; Eisenbarth, U. [GSI (Germany); Guilbaud, O. [Universite Paris Sud (France); Fils, J.; Goette, S. [GSI (Germany); Habib, J. [Universite Paris Sud (France); Hochhaus, D.; Javorkova, D. [GSI (Germany); Neumayer, P. [Extreme Matter Institute, EMMI (Germany); Kazamias, S.; Pittman, M.; Ros, D. [Universite Paris Sud (France); Seres, J.; Spielmann, Ch. [Friedrich Schiller-University (Germany); Zielbauer, B.; Zimmer, D. [GSI (Germany)

    2010-02-15

    Proposed as satellite-based weapons during the 1980s, X-ray lasing was for a long time only achieved with enormous amounts of pump energy in either nuclear explosions or at kilojoule-class laser installations. During the last few years a tremendous development was achieved, most visible in the realisation of the FEL lasers at DESY and SLAC. As important for a wider applicability is the enormous reduction in pump energy for laser pumped plasma X-ray lasers, which now brings such devices into the range of applications for diagnostics and spectroscopy even in smaller laboratories. Main developments were the transient excitation scheme and the optimized pumping concepts. This paper concentrates on developments at the GSI Helmholtzcenter at Darmstadt aiming towards reliable X-ray laser sources in the range from 50 to several 100 eV. The main driving forces for the laser development at GSI are the possible application for the spectroscopy of Li-like ions in the storage ring ESR and the future storage ring NESR at FAIR, and the interest in novel plasma diagnostics.

  12. Progress in the applicability of plasma X-ray lasers

    International Nuclear Information System (INIS)

    Kuehl, T.; Aurand, B.; Bagnoud, V.; Ecker, B.; Eisenbarth, U.; Guilbaud, O.; Fils, J.; Goette, S.; Habib, J.; Hochhaus, D.; Javorkova, D.; Neumayer, P.; Kazamias, S.; Pittman, M.; Ros, D.; Seres, J.; Spielmann, Ch.; Zielbauer, B.; Zimmer, D.

    2010-01-01

    Proposed as satellite-based weapons during the 1980s, X-ray lasing was for a long time only achieved with enormous amounts of pump energy in either nuclear explosions or at kilojoule-class laser installations. During the last few years a tremendous development was achieved, most visible in the realisation of the FEL lasers at DESY and SLAC. As important for a wider applicability is the enormous reduction in pump energy for laser pumped plasma X-ray lasers, which now brings such devices into the range of applications for diagnostics and spectroscopy even in smaller laboratories. Main developments were the transient excitation scheme and the optimized pumping concepts. This paper concentrates on developments at the GSI Helmholtzcenter at Darmstadt aiming towards reliable X-ray laser sources in the range from 50 to several 100 eV. The main driving forces for the laser development at GSI are the possible application for the spectroscopy of Li-like ions in the storage ring ESR and the future storage ring NESR at FAIR, and the interest in novel plasma diagnostics.

  13. On the theory of time-resolved x-ray diffraction

    DEFF Research Database (Denmark)

    Henriksen, Niels Engholm; Møller, Klaus Braagaard

    2008-01-01

    We derive the basic theoretical formulation for X-ray diffraction with pulsed fields, using a fully quantized description of light and matter. Relevant time scales are discussed for coherent as well as incoherent X-ray pulses, and we provide expressions to be used for calculation...... of the experimental diffraction signal for both types of X-ray sources. We present a simple analysis of time-resolved X-ray scattering for direct bond breaking in diatomic molecules. This essentially analytical approach highlights the relation between the signal and the time-dependent quantum distribution...

  14. Spatially resolved X-ray spectra of coronal active regions

    International Nuclear Information System (INIS)

    Catura, R.C.; Acton, L.W.; Joki, E.G.; Rapley, C.G.; Culhane, J.L.

    1975-01-01

    X-ray spectra from a number of coronal active regions were obtained during ATM support rocket flights carried out by the Lockheed group on June 11 and December 19, 1973. Multi-grid collimators were used to provide fields of view of 40ins. diameter and 90ins. diameter for a number of scanning crystal spectrometers and a bent crystal spectrometer which employed a position sensitive proportional counter to register the diffracted spectrum. A solar image was produced on film and on a TV camera on board the rocket with the aid of a 1 A Hα filter. A small part of the X-ray collimator was used to generate a multiple spot diffraction pattern which was superimposed on the Hα image and the composite picture was transmitted to the ground. Pre-launch calibrations allowed the spot corresponding to the X-ray collimator axis to be identified and so the collimator pointing direction on the solar disc was controlled from the ground by means of commands sent to the rocket. (Auth.)

  15. Temporally coherent x-ray laser with the high order harmonic light

    International Nuclear Information System (INIS)

    Hasegawa, Noboru; Kawachi, Tetsuya; Kishimoto, Maki; Sukegawa, Kouta; Tanaka, Momoko; Ochi, Yoshihiro; Nishikino, Masaharu; Kawazome, Hayato; Nagashima, Keisuke

    2005-01-01

    We obtained the neon-like manganese x-ray laser with the injection of the high order harmonic light as the seed x-ray at the wavelength of 26.9 nm for the purpose of generation of the temporally coherent x-ray laser. The x-ray amplifier, which has quite narrow spectral width, selected and amplified the temporally coherent mode of the harmonic light. The temporal coherence of the mode selected harmonic light was nearly transform limited pulse, and the obtained x-ray laser with the seed x-ray expected to be nearly temporally coherent x-ray. (author)

  16. Laser-driven soft-X-ray undulator source

    International Nuclear Information System (INIS)

    Fuchs, Matthias

    2010-01-01

    The experimental results described in this thesis demonstrate the successful synergy between the research fields described above: the development of an undulator source driven by laser-plasma accelerated electron beams. First efforts in this new field have led to the production of radiation in the visible to infrared part of the electromagnetic spectrum [Schlenvoigt et al., 2008]. In contrast to these early achievements, the experiment described here shows the successful production of laser-driven undulator radiation in the soft-X-ray range with a remarkable reproducibility. The source produced tunable, collimated beams with a wavelength of ∝17 nm from a compact setup. Undulator spectra were detected in ∝70% of consecutive driver-laser shots, which is a remarkable reproducibility for a first proof-of-concept demonstration using ultra-high intensity laser systems. This can be attributed to a stable electron acceleration scheme as well as to the first application of miniature magnetic quadrupole lenses with laseraccelerated beams. The lenses significantly reduce the electron beam divergence and its angular shot-to-shot fluctuations The setup of this experiment is the foundation of potential university-laboratory-sized, highly-brilliant hard X-ray sources. By increasing the electron energy to about 1 GeV, X-ray pulses with an expected duration of ∝10 fs and a photon energy of 1 keV could be produced in an almost identical arrangement. It can also be used as a testbed for the development of a free-electron laser of significantly smaller dimension than facilities based on conventional accelerators [Gruener et al., 2007]. Such compact sources have the potential for application in many fields of science. In addition, these developments could lead to ideal sources for ultrafast pump-probe experiments due to the perfect synchronization of the X-ray beam to the driver laser. (orig.)

  17. Laser-driven soft-X-ray undulator source

    Energy Technology Data Exchange (ETDEWEB)

    Fuchs, Matthias

    2010-08-04

    The experimental results described in this thesis demonstrate the successful synergy between the research fields described above: the development of an undulator source driven by laser-plasma accelerated electron beams. First efforts in this new field have led to the production of radiation in the visible to infrared part of the electromagnetic spectrum [Schlenvoigt et al., 2008]. In contrast to these early achievements, the experiment described here shows the successful production of laser-driven undulator radiation in the soft-X-ray range with a remarkable reproducibility. The source produced tunable, collimated beams with a wavelength of {proportional_to}17 nm from a compact setup. Undulator spectra were detected in {proportional_to}70% of consecutive driver-laser shots, which is a remarkable reproducibility for a first proof-of-concept demonstration using ultra-high intensity laser systems. This can be attributed to a stable electron acceleration scheme as well as to the first application of miniature magnetic quadrupole lenses with laseraccelerated beams. The lenses significantly reduce the electron beam divergence and its angular shot-to-shot fluctuations The setup of this experiment is the foundation of potential university-laboratory-sized, highly-brilliant hard X-ray sources. By increasing the electron energy to about 1 GeV, X-ray pulses with an expected duration of {proportional_to}10 fs and a photon energy of 1 keV could be produced in an almost identical arrangement. It can also be used as a testbed for the development of a free-electron laser of significantly smaller dimension than facilities based on conventional accelerators [Gruener et al., 2007]. Such compact sources have the potential for application in many fields of science. In addition, these developments could lead to ideal sources for ultrafast pump-probe experiments due to the perfect synchronization of the X-ray beam to the driver laser. (orig.)

  18. Time-resolved x-ray line emission studies of thermal transport in multiple beam uv-irradiated targets

    International Nuclear Information System (INIS)

    Jaanimagi, P.A.; Henke, B.L.; Delettrez, J.; Richardson, M.C.

    1984-01-01

    Thermal transport in spherical targets irradiated with multiple, nanosecond duration laser beams, has been a topic of much discussion recently. Different inferences on the level of thermal flux inhibition have been drawn from plasma velocity and x-ray spectroscopic diagnostics. We present new measurements of thermal transport on spherical targets made through time-resolved x-ray spectroscopic measurements of the progress of the ablation surface through thin layers of material on the surface of the target. These measurements, made with 6 and 12 uv (351 nm) nanosecond beams from OMEGA, will be compared to previous thermal transport measurements. Transparencies of the conference presentation are given

  19. PLEIADES: A picosecond Compton scattering x-ray source for advanced backlighting and time-resolved material studies

    International Nuclear Information System (INIS)

    Gibson, David J.; Anderson, Scott G.; Barty, Christopher P.J.; Betts, Shawn M.; Booth, Rex; Brown, Winthrop J.; Crane, John K.; Cross, Robert R.; Fittinghoff, David N.; Hartemann, Fred V.; Kuba, Jaroslav; Le Sage, Gregory P.; Slaughter, Dennis R.; Tremaine, Aaron M.; Wootton, Alan J.; Hartouni, Edward P.; Springer, Paul T.; Rosenzweig, James B.

    2004-01-01

    The PLEIADES (Picosecond Laser-Electron Inter-Action for the Dynamical Evaluation of Structures) facility has produced first light at 70 keV. This milestone offers a new opportunity to develop laser-driven, compact, tunable x-ray sources for critical applications such as diagnostics for the National Ignition Facility and time-resolved material studies. The electron beam was focused to 50 μm rms, at 57 MeV, with 260 pC of charge, a relative energy spread of 0.2%, and a normalized emittance of 5 mm mrad horizontally and 13 mm mrad vertically. The scattered 820 nm laser pulse had an energy of 180 mJ and a duration of 54 fs. Initial x rays were captured with a cooled charge-coupled device using a cesium iodide scintillator; the peak photon energy was approximately 78 keV, with a total x-ray flux of 1.3x10 6 photons/shot, and the observed angular distribution found to agree very well with three-dimensional codes. Simple K-edge radiography of a tantalum foil showed good agreement with the theoretical divergence-angle dependence of the x-ray energy. Optimization of the x-ray dose is currently under way, with the goal of reaching 10 8 photons/shot and a peak brightness approaching 10 20 photons/mm 2 /mrad 2 /s/0.1% bandwidth

  20. Time-resolved X-ray studies using third generation synchrotron radiation sources

    International Nuclear Information System (INIS)

    Mills, D.M.

    1991-10-01

    The third generation, high-brilliance, hard x-ray, synchrotron radiation (SR) sources currently under construction (ESRF at Grenoble, France; APS at Argonne, Illinois; and SPring-8 at Harima, Japan) will usher in a new era of x-ray experimentation for both physical and biological sciences. One of the most exciting areas of experimentation will be the extension of x-ray scattering and diffraction techniques to the study of transient or time-evolving systems. The high repetition rate, short-pulse duration, high brilliance, and variable spectral bandwidth of these sources make them ideal for x-ray time-resolved studies. The temporal properties (bunch length, interpulse period, etc.) of these new sources will be summarized. Finally, the scientific potential and the technological challenges of time-resolved x-ray scattering from these new sources will be described. 13 refs., 4 figs

  1. Investigating high speed phenomena in laser plasma interactions using dilation x-ray imager (invited).

    Science.gov (United States)

    Nagel, S R; Hilsabeck, T J; Bell, P M; Bradley, D K; Ayers, M J; Piston, K; Felker, B; Kilkenny, J D; Chung, T; Sammuli, B; Hares, J D; Dymoke-Bradshaw, A K L

    2014-11-01

    The DIlation X-ray Imager (DIXI) is a new, high-speed x-ray framing camera at the National Ignition Facility (NIF) sensitive to x-rays in the range of ≈2-17 keV. DIXI uses the pulse-dilation technique to achieve a temporal resolution of less than 10 ps, a ≈10× improvement over conventional framing cameras currently employed on the NIF (≈100 ps resolution), and otherwise only attainable with 1D streaked imaging. The pulse-dilation technique utilizes a voltage ramp to impart a velocity gradient on the signal-bearing electrons. The temporal response, spatial resolution, and x-ray sensitivity of DIXI are characterized with a short x-ray impulse generated using the COMET laser facility at Lawrence Livermore National Laboratory. At the NIF a pinhole array at 10 cm from target chamber center (tcc) projects images onto the photocathode situated outside the NIF chamber wall with a magnification of ≈64×. DIXI will provide important capabilities for warm-dense-matter physics, high-energy-density science, and inertial confinement fusion, adding important capabilities to temporally resolve hot-spot formation, x-ray emission, fuel motion, and mix levels in the hot-spot at neutron yields of up to 10(17). We present characterization data as well as first results on electron-transport phenomena in buried-layer foil experiments.

  2. Investigating high speed phenomena in laser plasma interactions using dilation x-ray imager (invited)

    Energy Technology Data Exchange (ETDEWEB)

    Nagel, S. R., E-mail: nagel7@llnl.gov; Bell, P. M.; Bradley, D. K.; Ayers, M. J.; Piston, K.; Felker, B. [Lawrence Livermore National Laboratory, 7000 East Avenue, Livermore, California 94550 (United States); Hilsabeck, T. J.; Kilkenny, J. D.; Chung, T.; Sammuli, B. [General Atomics, P.O. Box 85608, San Diego, California 92186-5608 (United States); Hares, J. D.; Dymoke-Bradshaw, A. K. L. [Kentech Instruments Ltd., Wallingford, Oxfordshire OX10 (United Kingdom)

    2014-11-15

    The DIlation X-ray Imager (DIXI) is a new, high-speed x-ray framing camera at the National Ignition Facility (NIF) sensitive to x-rays in the range of ≈2–17 keV. DIXI uses the pulse-dilation technique to achieve a temporal resolution of less than 10 ps, a ≈10× improvement over conventional framing cameras currently employed on the NIF (≈100 ps resolution), and otherwise only attainable with 1D streaked imaging. The pulse-dilation technique utilizes a voltage ramp to impart a velocity gradient on the signal-bearing electrons. The temporal response, spatial resolution, and x-ray sensitivity of DIXI are characterized with a short x-ray impulse generated using the COMET laser facility at Lawrence Livermore National Laboratory. At the NIF a pinhole array at 10 cm from target chamber center (tcc) projects images onto the photocathode situated outside the NIF chamber wall with a magnification of ≈64×. DIXI will provide important capabilities for warm-dense-matter physics, high-energy-density science, and inertial confinement fusion, adding important capabilities to temporally resolve hot-spot formation, x-ray emission, fuel motion, and mix levels in the hot-spot at neutron yields of up to 10{sup 17}. We present characterization data as well as first results on electron-transport phenomena in buried-layer foil experiments.

  3. X-ray free electron laser and its application to 3-dimensional imaging of non-crystalline nano-structure

    International Nuclear Information System (INIS)

    Ishikawa, Tetsuya

    2007-01-01

    The Laser in the X-ray region has been anticipated to be realized as a light source to probe the nano-world. Free electron lasers using high energy electron accelerators have been promising the candidates. The finding of the principle of Self-Amplified Spontaneous Emission (SASE) resolved the technological difficulties accompanying the X-ray free electron laser, and the construction of large scale SASE facilities started in western countries. In Japan the construction of an SASE facility started in 2006 to be completed in 2010 at the site of the large synchrotron radiation facility, SPring-8 positioned as a 'critical technology of national importance' by the Japanese government. The principle of the X-ray free electron laser is explained and the outline of the Japanese facility construction plan is presented. Also the application of the X-ray laser to the imaging of non-crystalline nano-structure is introduced. (K.Yoshida)

  4. X-ray calibration facility for plasma diagnostics of the MegaJoule laser

    International Nuclear Information System (INIS)

    Hubert, S.; Prevot, V.

    2013-01-01

    The Laser MegaJoule (LMJ) located at CEA-CESTA will be equipped with x-ray plasma diagnostics using different kinds of x-ray components such as filters, mirrors, crystals, detectors and cameras. To guarantee LMJ measurements, detectors such as x-ray cameras need to be regularly calibrated. An x-ray laboratory is devoted to this task and performs absolute x-ray calibrations for similar x-ray cameras running on Laser Integration Line (LIL). This paper presents the x-ray calibration bench with its x-ray tube based High Energy x-ray Source (HEXS) and some calibration results. By mean of an ingenious transposition system under vacuum absolute x-ray calibration of x-ray cameras, like streak and stripline ones, can be carried out. Coupled to a new collimation system with micrometric accuracy on aperture sensitivity quantum efficiency measurements can be achieved with reduced uncertainties. (authors)

  5. X-ray spectroscopy of laser imploded targets

    International Nuclear Information System (INIS)

    Yaakobi, B.; Skupsky, S.; McCrory, R.L.; Hooper, C.F.; Deckman, H.; Bourke, P.; Soures, J.M.

    1981-01-01

    X-ray spectroscopy provides a variety of means for studying the interaction of lasers with plasmas, in particular the interaction with imploding targets in inertial confinement fusion. A typical fusion target is composed of materials other than the thermonuclear fuel which play a variety of roles (tamping, shielding, thermal isolation, etc.). These structural elements emit characteristic X-ray lines and continua, and through their spectral and spatial distributions can yield very valuable information on the interaction and implosion dynamics. Examples are the study of heat conductivity, the mixing of different target layers, and the determination of temperature and density at the compressed target core. Results will be shown for electron densities Nsub(e) approximately equal to 10 24 cm -3 and temperatures T approximately equal to 1 keV measured during compression of argon-filled targets with a six-beam laser of peak power 2 TW. (author)

  6. X-ray absorption spectroscopy in the keV range with laser generated high harmonic radiation

    International Nuclear Information System (INIS)

    Seres, Enikoe; Seres, Jozsef; Spielmann, Christian

    2006-01-01

    By irradiating He and Ne atoms with 3 mJ, 12 fs, near infrared laser pulses from a tabletop laser system, the authors generated spatially and temporally coherent x rays up to a photon energy of 3.5 keV. With this source it is possible to use high-harmonic radiation for x-ray absorption spectroscopy in the keV range. They were able to clearly resolve the L absorption edges of titanium and copper and the K edges of aluminum and silicon. From the fine structure of the x-ray absorption they estimated the interatomic distances

  7. Harmonic lasing in x-ray free electron lasers

    Directory of Open Access Journals (Sweden)

    E. A. Schneidmiller

    2012-08-01

    Full Text Available Harmonic lasing in a free electron laser with a planar undulator (under the condition that the fundamental frequency is suppressed might be a cheap and efficient way of extension of wavelength ranges of existing and planned x-ray free electron laser (FEL facilities. Contrary to nonlinear harmonic generation, harmonic lasing can provide much more intense, stable, and narrow-band FEL beam which is easier to handle due to the suppressed fundamental frequency. In this paper we perform a parametrization of the solution of the eigenvalue equation for lasing at odd harmonics, and present an explicit expression for FEL gain length, taking into account all essential effects. We propose and discuss methods for suppression of the fundamental harmonic. We also suggest a combined use of harmonic lasing and lasing at the retuned fundamental wavelength in order to reduce bandwidth and to increase brilliance of x-ray beam at saturation. Considering 3rd harmonic lasing as a practical example, we come to the conclusion that it is much more robust than usually thought, and can be widely used in the existing or planned x-ray FEL (XFEL facilities. In particular, Linac Coherent Light Source (LCLS after a minor modification can lase to saturation at the 3rd harmonic up to the photon energy of 25–30 keV providing multigigawatt power level and narrow bandwidth. As for the European XFEL, harmonic lasing would allow one to extend operating range (ultimately up to 100 keV, to reduce FEL bandwidth and to increase brilliance, to enable two-color operation for pump-probe experiments, and to provide more flexible operation at different electron energies. Similar improvements can be realized in other x-ray FEL facilities with gap-tunable undulators like FLASH II, SACLA, LCLS II, etc. Harmonic lasing can be an attractive option for compact x-ray FELs (driven by electron beams with a relatively low energy, allowing the use of the standard undulator technology instead of

  8. Time response characteristics of X-ray detector system on Silex-Ⅰ laser facility

    International Nuclear Information System (INIS)

    Yi Rongqing; He Xiao'an; Li Hang; Du Huabing; Zhang Haiying; Cao Zhurong

    2013-01-01

    On the Silex-Ⅰ laser facility, the time response characteristics of XRD detector were studied. A laser with a pulse of 32 fs and a wavelength of 800 nm was used to irradiate a plane Au target. X-ray calibrated method of time of exposure X-ray framing camera and time resolution of X-ray streak camera was explored. The time response characteristics of XRD detector and time process of X-ray emission were obtained from experiment. We obtained X-ray calibration method of time of exposure X-ray framing camera and time resolution of X-ray streak camera. (authors)

  9. Probing Photoinduced Structural Phase Transitions by Fast or Ultra-Fast Time-Resolved X-Ray Diffraction

    Science.gov (United States)

    Cailleau, Hervé Collet, Eric; Buron-Le Cointe, Marylise; Lemée-Cailleau, Marie-Hélène Koshihara, Shin-Ya

    A new frontier in the field of structural science is the emergence of the fast and ultra-fast X-ray science. Recent developments in time-resolved X-ray diffraction promise direct access to the dynamics of electronic, atomic and molecular motions in condensed matter triggered by a pulsed laser irradiation, i.e. to record "molecular movies" during the transformation of matter initiated by light pulse. These laser pump and X-ray probe techniques now provide an outstanding opportunity for the direct observation of a photoinduced structural phase transition as it takes place. The use of X-ray short-pulse of about 100ps around third-generation synchrotron sources allows structural investigations of fast photoinduced processes. Other new X-ray sources, such as laser-produced plasma ones, generate ultra-short pulses down to 100 fs. This opens the way to femtosecond X-ray crystallography, but with rather low X-ray intensities and more limited experimental possibilities at present. However this new ultra-fast science rapidly progresses around these sources and new large-scale projects exist. It is the aim of this contribution to overview the state of art and the perspectives of fast and ultra-fast X-ray scattering techniques to study photoinduced phase transitions (here, the word ultra-fast is used for sub-picosecond time resolution). In particular we would like to largely present the contribution of crystallographic methods in comparison with optical methods, such as pump-probe reflectivity measurements, the reader being not necessary familiar with X-ray scattering. Thus we want to present which type of physical information can be obtained from the positions of the Bragg peaks, their intensity and their shape, as well as from the diffuse scattering beyond Bragg peaks. An important physical feature is to take into consideration the difference in nature between a photoinduced phase transition and conventional homogeneous photoinduced chemical or biochemical processes where

  10. Synchronization of x-ray pulses to the pump laser in an ultrafast x-ray facility

    International Nuclear Information System (INIS)

    Corlett, J.N.; Barry, W.; Byrd, J.M.; Schoenlein, R.; Zholents, A.

    2002-01-01

    Accurate timing of ultrafast x-ray probe pulses emitted from a synchrotron radiation source with respect to a pump laser exciting processes in the sample under study is critical for the investigation of structural dynamics in the femtosecond regime. We describe a scheme for synchronizing femtosecond x-ray pulses relative to a pump laser. X-ray pulses of <100 fs duration are generated from a proposed source based on a recirculating superconducting linac [1,2,3]. Short x-ray pulses are obtained by a process of electron pulse compression, followed by transverse temporal correlation of the electrons, and ultimately x-ray pulse compression. Timing of the arrival of the x-ray pulse with respect to the pump laser is found to be dominated by the operation of the deflecting cavities which provide the transverse temporal correlation of the electrons. The deflecting cavities are driven from a highly stable RF signal derived from a modelocked laser oscillator which is also the origin of the pump l aser pulses

  11. Time-resolved materials science opportunities using synchrotron x-ray sources

    International Nuclear Information System (INIS)

    Larson, B.C.; Tischler, J.Z.

    1995-06-01

    The high brightness, high intensity, and pulsed time-structure of synchrotron sources provide new opportunities for time-resolved x-ray diffraction investigations. With third generation synchrotron sources coming on line, high brilliance and high brightness are now available in x-ray beams with the highest flux. In addition to the high average flux, the instantaneous flux available in synchrotron beams is greatly enhanced by the pulsed time structure, which consists of short bursts of x-rays that are separated by ∼tens to hundreds of nanoseconds. Time-resolved one- and two-dimensional position sensitive detection techniques that take advantage of synchrotron radiation for materials science x-ray diffraction investigations are presented, and time resolved materials science applications are discussed in terms of recent diffraction and spectroscopy results and materials research opportunities

  12. Time resolved x-ray photography of a dense plasma focus

    International Nuclear Information System (INIS)

    Burnett, J.C.; Meyer, J.; Rankin, G.

    1977-01-01

    The temporal development of the hot plasma in a dense plasma focus is studied by x-ray streak photography of approximately 2 ns resolution time. It is shown that initially a uniform x-ray emitting pinch plasma is formed which subsequently cools down until x-ray emission stops after approximately 50 ns. At a time of around 100 ns after initial x-ray emission coinciding with the break-up time of the pinch a second burst of x-rays is observed coming from small localized regions. The observations are compared with results obtained from time-resolved shadow and schlieren photography of a similar dense focus discharge. (author)

  13. Hydrodynamic aspects of selenium X-ray laser targets

    Energy Technology Data Exchange (ETDEWEB)

    Charatis, G; Busch, G E; Shepard, C L; Campbell, P M; Rosen, M D

    1986-10-01

    Recent experiments at KMS have been performed to investigate parameter variations of target component thickness, laser pulse duration and intensity, and one-sided vs two-sided irradiation in order to optimize the performance of the Livermore exploding foil selenium x-ray laser experiments. Preliminary experiments with selenium double foil targets were also conducted as a means of prolonging the duration and enlarging the spatial extent of the lasing conditions. Four-frame holographic interferometry was used in determining the time-dependence of density profiles obtained by Abel inversion of the interferometric fringe field and comparisons were made to LASNEX code calculations.

  14. Beamline for X-ray Free Electron Laser of SACLA

    International Nuclear Information System (INIS)

    Tono, K; Togashi, T; Ohashi, H; Kimura, H; Takahashi, S; Takeshita, K; Tomizawa, H; Goto, S; Inubushi, Y; Sato, T; Yabashi, M

    2013-01-01

    A beamline for X-ray free electron laser (XFEL) has been developed at SACLA, SPring-8 Angstrom Compact free electron LAser. The beamline delivers and diagnoses an XFEL beam without degrading the beam quality. The transport optics are applicable in the range of 4–30 keV with a double-crystal monochromator or 4–15 keV with either of two double-mirror systems. A photon diagnostic system of the beamline monitors intensity, photon energy, center-of-mass position, and spatial profile in shot-by-shot and non-destructive manners.

  15. Development of x-ray laser and its application

    Energy Technology Data Exchange (ETDEWEB)

    Kawachi, Tetsuya; Kado, Masataka; Hasegawa, Noboru [Japan Atomic Energy Research Inst., Kizu, Kyoto (Japan). Kansai Research Establishment] [and others

    2001-10-01

    Nickel-like silver and tin X-ray lasers (XRL) at wavelengths of 13.9 nm and 11.9 nm, respectively, in the transient collisional-excitation scheme. The gain-length product is 10 for the former case and 8.4 for the latter. The size of the gain region and the beam divergence of the silver laser are measured to be 75 {mu}m x 25 {mu}m and about 6 mrad, respectively. Our plans in the near future, which are applications of XRL, generation of XRL with high spatial coherence and short-wavelength XRL, are also shown. (author)

  16. X-ray refractive index of laser-dressed atoms

    OpenAIRE

    Buth, Christian; Santra, Robin

    2008-01-01

    We investigated the complex index of refraction in the x-ray regime of atoms in laser light. The laser (intensity up to 10^13 W/cm^2, wavelength 800nm) modifies the atomic states but, by assumption, does not excite or ionize the atoms in their electronic ground state. Using quantum electrodynamics, we devise an ab initio theory to calculate the dynamic dipole polarizability and the photoabsorption cross section, which are subsequently used to determine the real and imaginary part, respectivel...

  17. Development of x-ray laser and its application

    International Nuclear Information System (INIS)

    Kawachi, Tetsuya; Kado, Masataka; Hasegawa, Noboru

    2001-01-01

    Nickel-like silver and tin X-ray lasers (XRL) at wavelengths of 13.9 nm and 11.9 nm, respectively, in the transient collisional-excitation scheme. The gain-length product is 10 for the former case and 8.4 for the latter. The size of the gain region and the beam divergence of the silver laser are measured to be 75 μm x 25 μm and about 6 mrad, respectively. Our plans in the near future, which are applications of XRL, generation of XRL with high spatial coherence and short-wavelength XRL, are also shown. (author)

  18. Recent developments in x-ray laser research at LLE

    International Nuclear Information System (INIS)

    Boehly, T.; Yaakobi, B.; Craxton, R.S.; Epstein, R.; Richardson, M.C.; Russotto, M.; Soures, J.M.; Wang, J.

    1989-01-01

    The authors present results and analysis of recent experiments using multiple-foil target designs for a collisional excitation x-ray laser in Ne-like nickel and germanium. These targets, which are designed to yield higher gains than single-exploding-foil targets, are irradiated by 600 ps pulses of 351 nm light in a single 18-mm line from GDL. The lasing lines at --230 A are observed with a 1-m grazing incidence grating spectrometer. They discuss the relative merit of different pump-laser wavelengths and present experimental results for three wavelengths: 1.06 μm, 527 nm, and 351 nm. They present plans for the conversion of the GDL laser to a --100 J - 10 ps laser (10 TW) which will be used for producing a recombinationally pumped laser in Al which is predicted to lase at 39 A. Results of computer simulation of these proposed experiments are presented

  19. Batch crystallization of rhodopsin for structural dynamics using an X-ray free-electron laser

    Energy Technology Data Exchange (ETDEWEB)

    Wu, Wenting; Nogly, Przemyslaw; Rheinberger, Jan; Kick, Leonhard M.; Gati, Cornelius; Nelson, Garrett; Deupi, Xavier; Standfuss, Jörg; Schertler, Gebhard; Panneels, Valérie, E-mail: valerie.panneels@psi.ch [Paul Scherrer Institute, OFLC/103, 5232 Villigen-PSI (Switzerland)

    2015-06-27

    A new batch preparation method is presented for high-density micrometre-sized crystals of the G protein-coupled receptor rhodopsin for use in time-resolved serial femtosecond crystallography at an X-ray free-electron laser using a liquid jet. Rhodopsin is a membrane protein from the G protein-coupled receptor family. Together with its ligand retinal, it forms the visual pigment responsible for night vision. In order to perform ultrafast dynamics studies, a time-resolved serial femtosecond crystallography method is required owing to the nonreversible activation of rhodopsin. In such an approach, microcrystals in suspension are delivered into the X-ray pulses of an X-ray free-electron laser (XFEL) after a precise photoactivation delay. Here, a millilitre batch production of high-density microcrystals was developed by four methodical conversion steps starting from known vapour-diffusion crystallization protocols: (i) screening the low-salt crystallization conditions preferred for serial crystallography by vapour diffusion, (ii) optimization of batch crystallization, (iii) testing the crystal size and quality using second-harmonic generation (SHG) imaging and X-ray powder diffraction and (iv) production of millilitres of rhodopsin crystal suspension in batches for serial crystallography tests; these crystals diffracted at an XFEL at the Linac Coherent Light Source using a liquid-jet setup.

  20. Time-Resolved Soft X-ray Diffraction Reveals Transient Structural Distortions of Ternary Liquid Crystals

    Directory of Open Access Journals (Sweden)

    Klaus Mann

    2009-11-01

    Full Text Available Home-based soft X-ray time-resolved scattering experiments with nanosecond time resolution (10 ns and nanometer spatial resolution were carried out at a table top soft X-ray plasma source (2.2–5.2 nm. The investigated system was the lyotropic liquid crystal C16E7/paraffin/glycerol/formamide/IR 5. Usually, major changes in physical, chemical, and/or optical properties of the sample occur as a result of structural changes and shrinking morphology. Here, these effects occur as a consequence of the energy absorption in the sample upon optical laser excitation in the IR regime. The liquid crystal shows changes in the structural response within few hundred nanoseconds showing a time decay of 182 ns. A decrease of the Bragg peak diffracted intensity of 30% and a coherent macroscopic movement of the Bragg reflection are found as a response to the optical pump. The Bragg reflection movement is established to be isotropic and diffusion controlled (1 μs. Structural processes are analyzed in the Patterson analysis framework of the time-varying diffraction peaks revealing that the inter-lamellar distance increases by 2.7 Å resulting in an elongation of the coherently expanding lamella crystallite. The present studies emphasize the possibility of applying TR-SXRD techniques for studying the mechanical dynamics of nanosystems.

  1. A compact x-ray free electron laser

    International Nuclear Information System (INIS)

    Barletta, W.; Attac, M.; Cline, D.B.

    1988-01-01

    We present a design concept and simulation of the performance of a compact x-ray, free electron laser driven by ultra-high gradient rf-linacs. The accelerator design is based on recent advances in high gradient technology by a LLNL/SLAC/LBL collaboration and on the development of bright, high current electron sources by BNL and LANL. The GeV electron beams generated with such accelerators can be concerted to soft x-rays in the range from 2--10 nm by passage through short period, high fields strength wigglers as are being designed at Rocketdyne. Linear light sources of this type can produce trains of picosecond (or shorter) pulses of extremely high spectral brilliance suitable for flash holography of biological specimens in vivo and for studies of fast chemical reactions. 12 refs., 8 figs., 4 tabs

  2. Spatially resolved single crystal x-ray spectropolarimetry of wire array z-pinch plasmas.

    Science.gov (United States)

    Wallace, M S; Haque, S; Neill, P; Pereira, N R; Presura, R

    2018-01-01

    A recently developed single-crystal x-ray spectropolarimeter has been used to record paired sets of polarization-dependent and axially resolved x-ray spectra emitted by wire array z-pinches. In this measurement, two internal planes inside a suitable crystal diffract the x-rays into two perpendicular directions that are normal to each other, thereby separating incident x-rays into their linearly polarized components. This paper gives considerations for fielding the instrument on extended sources. Results from extended sources are difficult to interpret because generally the incident x-rays are not separated properly by the crystal. This difficulty is mitigated by using a series of collimating slits to select incident x-rays that propagate in a plane of symmetry between the polarization-splitting planes. The resulting instrument and some of the spatially resolved polarized x-ray spectra recorded for a 1-MA aluminum wire array z-pinch at the Nevada Terawatt Facility at the University of Nevada, Reno will be presented.

  3. The x-ray laser coherence experiments in neon-like yttrium

    International Nuclear Information System (INIS)

    Shimkaveg, G.M.; Carter, M.R.; Walling, R.S.; Ticehurst, J.M.; Koch, J.A.; Mrowka, S.; Trebes, J.E.; MacGowan, B.J.; Da Silva, L.B.; Matthews, D.L.; London, R.A.; Stewart, R.E.

    1992-01-01

    We present recent results from neon-like x-ray laser experiments conducted at the Nova laser's Two-Beam Facility. This begins a series of experiments aimed at the characterization and control of the degree of spatial coherece in our soft x-ray laser beams, important to planned applications areas susch as microscopy and holography. New instrumentation developed for this effort include a fully time-resolved coherence diagnostic (which records a multiple-slit diffraction pattern) and wide-angle extreme ultraviolet spectrographs and beam divergence cameras. We present new measurements of beam profiles and gain, as well as spatial coherence data such as time-resolved multi-slit diffraction patterns. This new time-resolved coherence data exhibit aperture functions which increase in size during the time of the lasing. Also, some preliminary data is given from the first ''double-foil'' experiments, involving two x-ray amplifiers spatially separated by 29 cm and shot sequentially, in an ''oscillator-amplifier'' configuration

  4. Imaging Macromolecules with X-ray laser pulses

    CERN Multimedia

    CERN. Geneva

    2017-01-01

    The short wavelength of X-rays allows us to resolve atoms, but in practise for biological materials the achievable resolution is limited by the destruction of the sample by the radiation that forms the image.  For over 100 years, the workaround to this problem of radiation damage has been to average signals from repeating copies of the object arranged in a large crystal.  It is now possible to overcome damage limits by using intense X-ray pulses that vaporise the sample, but which are short enough in duration to freeze any motion of the sample on the atomic scale.  With the advent of X-ray FELs we have been able to confirm this principle, and are now applying it to overcoming a major bottleneck for protein crystallography, which is the need for large well-diffracting crystals.  The intense pulses also open up opportunities to help solve the crystallographic phase problem.  In particular we have found that commonly-occurring disordered crystals that are usually not ...

  5. kHz femtosecond laser-plasma hard X-ray and fast ion source

    International Nuclear Information System (INIS)

    Thoss, A.; Korn, G.; Stiel, H.; Voigt, U.; Elsaesser, T.; Richardson, M.C.; Siders, C.W.; Faubel, M.

    2002-01-01

    We describe the first demonstration of a new stable, kHz femtosecond laser-plasma source of hard x-ray continuum and K α emission using a thin liquid metallic jet target. kHz femtosecond x-ray sources will find many applications in time-resolved x-ray diffraction and microscopy studies. As high intensity lasers become more compact and operate at increasingly high repetition-rates, they require a target configuration that is both repeatable from shot-to-shot and is debris-free. We have solved this requirement with the use of a fine (10-30 μm diameter) liquid metal jet target that provides a pristine, unperturbed filament surface at rates >100 kHz. A number of liquid metal targets are considered. We will show hard x-ray spectra recorded from liquid Ga targets that show the generation of the 9.3 keV and 10.3 keV, K α and K β lines superimposed on a multi-keV Bremsstrahlung continuum. This source was generated by a 50fs duration, 1 kHz, 2W, high intensity Ti:Sapphire laser. We will discuss the extension of this source to higher powers and higher repetition rates, providing harder x-ray emission, with the incorporation of pulse-shaping and other techniques to enhance the x-ray conversion efficiency. Using the same liquid target technology, we have also demonstrated the generation of forward-going sub-MeV protons from a 10 μm liquid water target at 1 kHz repetition rates. kHz sources of high energy ions will find many applications in time-resolved particle interaction studies, as well as lead to the efficient generation of short-lived isotopes for use in nuclear medicine and other applications. The protons were detected with CR-39 track detectors both in the forward and backward directions up to energies of ∼500 keV. As the intensity of compact high repetition-rate lasers sources increase, we can expect improvements in the energy, conversion efficiency and directionality to occur. The impact of these developments on a number of fields will be discussed. As compact

  6. Laser-driven x-ray and neutron source development for industrial applications of plasma accelerators

    Science.gov (United States)

    Brenner, C. M.; Mirfayzi, S. R.; Rusby, D. R.; Armstrong, C.; Alejo, A.; Wilson, L. A.; Clarke, R.; Ahmed, H.; Butler, N. M. H.; Haddock, D.; Higginson, A.; McClymont, A.; Murphy, C.; Notley, M.; Oliver, P.; Allott, R.; Hernandez-Gomez, C.; Kar, S.; McKenna, P.; Neely, D.

    2016-01-01

    Pulsed beams of energetic x-rays and neutrons from intense laser interactions with solid foils are promising for applications where bright, small emission area sources, capable of multi-modal delivery are ideal. Possible end users of laser-driven multi-modal sources are those requiring advanced non-destructive inspection techniques in industry sectors of high value commerce such as aerospace, nuclear and advanced manufacturing. We report on experimental work that demonstrates multi-modal operation of high power laser-solid interactions for neutron and x-ray beam generation. Measurements and Monte Carlo radiation transport simulations show that neutron yield is increased by a factor ~2 when a 1 mm copper foil is placed behind a 2 mm lithium foil, compared to using a 2 cm block of lithium only. We explore x-ray generation with a 10 picosecond drive pulse in order to tailor the spectral content for radiography with medium density alloy metals. The impact of using  >1 ps pulse duration on laser-accelerated electron beam generation and transport is discussed alongside the optimisation of subsequent bremsstrahlung emission in thin, high atomic number target foils. X-ray spectra are deconvolved from spectrometer measurements and simulation data generated using the GEANT4 Monte Carlo code. We also demonstrate the unique capability of laser-driven x-rays in being able to deliver single pulse high spatial resolution projection imaging of thick metallic objects. Active detector radiographic imaging of industrially relevant sample objects with a 10 ps drive pulse is presented for the first time, demonstrating that features of 200 μm size are resolved when projected at high magnification.

  7. Laser-driven x-ray and neutron source development for industrial applications of plasma accelerators

    International Nuclear Information System (INIS)

    Brenner, C M; Rusby, D R; Armstrong, C; Wilson, L A; Clarke, R; Haddock, D; McClymont, A; Notley, M; Oliver, P; Allott, R; Hernandez-Gomez, C; Neely, D; Mirfayzi, S R; Alejo, A; Ahmed, H; Kar, S; Butler, N M H; Higginson, A; McKenna, P; Murphy, C

    2016-01-01

    Pulsed beams of energetic x-rays and neutrons from intense laser interactions with solid foils are promising for applications where bright, small emission area sources, capable of multi-modal delivery are ideal. Possible end users of laser-driven multi-modal sources are those requiring advanced non-destructive inspection techniques in industry sectors of high value commerce such as aerospace, nuclear and advanced manufacturing. We report on experimental work that demonstrates multi-modal operation of high power laser-solid interactions for neutron and x-ray beam generation. Measurements and Monte Carlo radiation transport simulations show that neutron yield is increased by a factor ∼2 when a 1 mm copper foil is placed behind a 2 mm lithium foil, compared to using a 2 cm block of lithium only. We explore x-ray generation with a 10 picosecond drive pulse in order to tailor the spectral content for radiography with medium density alloy metals. The impact of using  >1 ps pulse duration on laser-accelerated electron beam generation and transport is discussed alongside the optimisation of subsequent bremsstrahlung emission in thin, high atomic number target foils. X-ray spectra are deconvolved from spectrometer measurements and simulation data generated using the GEANT4 Monte Carlo code. We also demonstrate the unique capability of laser-driven x-rays in being able to deliver single pulse high spatial resolution projection imaging of thick metallic objects. Active detector radiographic imaging of industrially relevant sample objects with a 10 ps drive pulse is presented for the first time, demonstrating that features of 200 μm size are resolved when projected at high magnification. (paper)

  8. High resolution X-ray spectromicroscopy of laser produced plasmas

    Energy Technology Data Exchange (ETDEWEB)

    Faenov, A.Ya. [Multi-charged Ions Spectra Data Center of VNIIFTRI (MISDC), Mendeleevo, Moscow region, (Russian Federation)

    2000-01-01

    In recent years new classes of X-ray spectroscopic instruments possessing both dispersive and focusing properties have been manufactured. Their principal advantage over more traditional instruments is that they combine very high luminosity with high spatial resolution, while preserving the highest possible spectral resolution of their dispersive elements. These instruments opened up the registration of plasmas in new regimes and surroundings. The measurements delivered new information about the properties of even previously studied traditional plasma objects (e.g. ns-laser produced plasmas). Also the detailed investigation of relatively new plasma laboratory sources with very small dimensions and low energy content (e.g. mJ fs-laser pulses) became possible. The purpose of this report is to give a short review of the experimental and theoretical results obtained in the past few years by MISDC (Multi-charged Ions Spectra Data Center) research team in the field of X-ray spectroscopy of a laser-produced plasma. Experimental spectra have been obtained at various laser installations with nanosecond, sub-nanosecond, picosecond and sub-picosecond pulses interacting with solid, gaseous or cluster targets in collaborations with research teams from Russia, USA, Germany, France, Poland, Belgium, Italy, China and Israel. Practically all results have been obtained with the help of spectrographs with spherically bent mica crystals operating in FSSR-1D, 2D schemes. (author)

  9. A split-beam probe-pump-probe scheme for femtosecond time resolved protein X-ray crystallography

    Directory of Open Access Journals (Sweden)

    Jasper J. van Thor

    2015-01-01

    Full Text Available In order to exploit the femtosecond pulse duration of X-ray Free-Electron Lasers (XFEL operating in the hard X-ray regime for ultrafast time-resolved protein crystallography experiments, critical parameters that determine the crystallographic signal-to-noise (I/σI must be addressed. For single-crystal studies under low absorbed dose conditions, it has been shown that the intrinsic pulse intensity stability as well as mode structure and jitter of this structure, significantly affect the crystallographic signal-to-noise. Here, geometrical parameters are theoretically explored for a three-beam scheme: X-ray probe, optical pump, X-ray probe (or “probe-pump-probe” which will allow experimental determination of the photo-induced structure factor amplitude differences, ΔF, in a ratiometric manner, thereby internally referencing the intensity noise of the XFEL source. In addition to a non-collinear split-beam geometry which separates un-pumped and pumped diffraction patterns on an area detector, applying an additional convergence angle to both beams by focusing leads to integration over mosaic blocks in the case of well-ordered stationary protein crystals. Ray-tracing X-ray diffraction simulations are performed for an example using photoactive yellow protein crystals in order to explore the geometrical design parameters which would be needed. The specifications for an X-ray split and delay instrument that implements both an offset angle and focused beams are discussed, for implementation of a probe-pump-probe scheme at the European XFEL. We discuss possible extension of single crystal studies to serial femtosecond crystallography, particularly in view of the expected X-ray damage and ablation due to the first probe pulse.

  10. Time-Resolved Small-Angle X-Ray Scattering

    NARCIS (Netherlands)

    ten Elshof, Johan E.; Besselink, R.; Stawski, Tomasz; Castricum, H.L.; Levy, D.; Zayat, M.

    2015-01-01

    This chapter focuses on time-resolved studies of nanostructure development in sol-gel liquids, that is, diluted sols, wet gels, and drying thin fffilms. The most commonly investigated classes of sol-gel materials are silica, organically modified silica, template-directed mesostructured silica,

  11. Development of small scale soft x-ray lasers: Aspects of data interpretation

    International Nuclear Information System (INIS)

    Skinner, C.H.; Kim, D.; Voorhees, D.; Suckewer, S.

    1990-02-01

    The widespread application of soft x-ray laser technology is contingent on the development of small scale soft x-ray lasers that do not require large laser facilities. Progress in the development of soft x-ray lasers pumped by a Nd laser of energy 6-12J is reported below. Some aspects of data interpretation and gain measurements in such systems are discussed. 11 refs., 11 figs

  12. Aerosol Imaging with a Soft X-ray Free Electron Laser

    International Nuclear Information System (INIS)

    Bogan, Michael J.; Boutet, Sebastien; Chapman, Henry N.; Marchesini, Stefano; Barty, Anton; Benner, W. Henry; Rohner, Urs; Frank, Matthias; Hau-Riege, Stefan P.; Bajt, Sasa; Woods, Bruce; Seibert, M.M.; Iwan, Bianca; Timneanu, Nicusor; Hajdu, Janos; Schulz, Joachim

    2010-01-01

    Lasers have long played a critical role in the advancement of aerosol science. A new regime of ultrafast laser technology has recently be realized, the world's first soft xray free electron laser. The Free electron LASer in Hamburg, FLASH, user facility produces a steady source of 10 femtosecond pulses of 7-32 nm x-rays with 10 12 photons per pulse. The high brightness, short wavelength, and high repetition rate (>500 pulses per second) of this laser offers unique capabilities for aerosol characterization. Here we use FLASH to perform the highest resolution imaging of single PM2.5 aerosol particles in flight to date. We resolve to 35 nm the morphology of fibrous and aggregated spherical carbonaceous nanoparticles that existed for less than two milliseconds in vacuum. Our result opens the possibility for high spatialand time-resolved single particle aerosol dynamics studies, filling a critical technological need in aerosol science.

  13. X-ray photoelectron microscope with a compact x-ray source generated by line-focused laser irradiation

    International Nuclear Information System (INIS)

    Yamaguchi, N.; Okamoto, Y.; Hara, T.; Takahashi, Z.; Nishimura, Y.; Sakata, A.; Watanabe, K.; Azuma, H.

    2004-01-01

    Full text: A laboratory-sized microscopic system of x-ray photoelectrons has been developing using a compact x-ray source produced by line-focused laser irradiation. The system is a scanning type photoelectron microscope where x-ray beam is micro-focused via a Schwartzschild optics. A compact laser-plasma x-ray source has been developed with a YAG laser system, a line-focus lens system, a tape-target driving system and a debris prevention system, that was operated at repetition rate of 10 Hz or 50 Hz. X-rays were delivered along line plasma whose length was 0.6 to 11 mm with higher intensity than that from a point-focused source. Because the transition line of Al V (13.1 nm) was prominent in the soft x-ray spectrum when the Al tape target irradiated at the lower power density of 10 11 W/cm 2 , the 13.1 nm x-ray was used as an excitation source. The Schwartzschild optics was set on the beamline at a distance about 1 m from the source, which was coated with Mo/Si multilayers for 13.1 nm x-ray. The designed demagnification is 224 that was confirmed in the previous experiment. Therefore, an x-ray micro spot of sub-micron size can be formed on a sample surface when the source size is less than about 0.2 mm. Samples were set on a two-axis high-precision piezo stage mounted to a four-axis manipulator. The electron energy analyzer was a spherical capacitor analyzer with mean diameter of 279.4 mm. The electron detector was a microchannel plate (MCP) with a phosphor screen and the optical image of electrons on the exit plane of the analyzer was taken and recorded by using an ultra low dark noise CCD camera, that was suited for detection of vast photoelectrons excited by x-ray pulse of ns-order duration. We performed spatial resolution test measurements by using a GaAs wafer coated with photo-resist that formed a stripe pattern. The spatial resolution less than 3 micron has been obtained from the variation of As 3d electron intensity along the position of the GaAs sample

  14. High resolution X-ray spectroscopy of laser generated plasmas

    International Nuclear Information System (INIS)

    Faenov, A.Ya.; Skobelev, I.Yu.; Rosmej, F.B.

    1999-01-01

    The application of recently developed spectroscopic instruments in laser produced plasmas with simultaneous high spectral and spatial resolution combined with high luminosity discovered new types of X-ray spectra. These new types are characterised by the disappearance of the resonance lines and the strong emission of dielectronic satellite spectra. Several types of transitions of highly charged ions are discovered which are unknown from usual sources employed in atomic physics. New theoretical models are developed and successfully applied for the interpretation and for plasma diagnostics. (orig.)

  15. High resolution X-ray spectroscopy of laser generated plasmas

    Energy Technology Data Exchange (ETDEWEB)

    Faenov, A.Ya.; Skobelev, I.Yu. [Multicharged Ions Spectra Data Center of VNIIFTRI, Mendeleevo (Russian Federation); Rosmej, F.B. [Technische Hochschule Darmstadt (Germany). Inst. fuer Kernphysik

    1999-11-01

    The application of recently developed spectroscopic instruments in laser produced plasmas with simultaneous high spectral and spatial resolution combined with high luminosity discovered new types of X-ray spectra. These new types are characterised by the disappearance of the resonance lines and the strong emission of dielectronic satellite spectra. Several types of transitions of highly charged ions are discovered which are unknown from usual sources employed in atomic physics. New theoretical models are developed and successfully applied for the interpretation and for plasma diagnostics. (orig.) 28 refs.

  16. Characterization of transient gain x-ray lasers

    International Nuclear Information System (INIS)

    Dunn, J.; Osterheld, A.; Shlyaptsev, V.

    1999-01-01

    We have performed numerical simulations of the transient collisional excitation Ni-like Pd 4d → 4p J = 0 → 1 147 angstrom laser transition recently observed at Lawrence Livermore National Laboratory (LLNL). The high gain ∼35 cm results from the experiment are compared with detailed modeling simulations from the 1-D RADEX code in order to better understand the main physics issues affecting the measured gain and x-ray laser propagation along the plasma column. Simulations indicate that the transient gain lifetime associated with the short pulse pumping and refraction of the x-ray laser beam out of the gain region are the main detrimental effects. Gain lifetimes of ∼7 ps(1/e decay) are inferred from the smoothly changing gain experimental observations and are in good agreement with the simulations. Furthermore, the modeling results indicate the presence of a longer-lived but lower gain later in time associated with the transition from transient to quasi-steady state excitation

  17. X-ray preionization for electric discharge lasers

    International Nuclear Information System (INIS)

    Lin, S.; Levatter, J.I.

    1979-01-01

    Using x rays of 60--200-keV photon energy (lambdaapprox.0.06--0.2 A) as an ionizing radiation source in a transmission-line-driven low-inductance discharge chamber, we have succeeded in generating spatially homogeneous pulsed avalanche discharges of several liter volume at greater than 1 atm pressure for up to 100-nsec duration. In concurrent laser generation experiments with relatively lossy windows, we have observed high-optical-quality pulsed uv laser output of up to 2 J/liter from such discharges in rare-gas/halogen mixtures, and IR laser output of up to 12.5 J/liter from a He/N 2 /CO 2 mixture

  18. Thin film growth studies using time-resolved x-ray scattering

    Science.gov (United States)

    Kowarik, Stefan

    2017-02-01

    Thin-film growth is important for novel functional materials and new generations of devices. The non-equilibrium growth physics involved is very challenging, because the energy landscape for atomic scale processes is determined by many parameters, such as the diffusion and Ehrlich-Schwoebel barriers. We review the in situ real-time techniques of x-ray diffraction (XRD), x-ray growth oscillations and diffuse x-ray scattering (GISAXS) for the determination of structure and morphology on length scales from Å to µm. We give examples of time resolved growth experiments mainly from molecular thin film growth, but also highlight growth of inorganic materials using molecular beam epitaxy (MBE) and electrochemical deposition from liquids. We discuss how scaling parameters of rate equation models and fundamental energy barriers in kinetic Monte Carlo methods can be determined from fits of the real-time x-ray data.

  19. Chandra Resolves Cosmic X-ray Glow and Finds Mysterious New Sources

    Science.gov (United States)

    2000-01-01

    While taking a giant leap towards solving one of the greatest mysteries of X-ray astronomy, NASA's Chandra X-ray Observatory also may have revealed the most distant objects ever seen in the universe and discovered two puzzling new types of cosmic objects. Not bad for being on the job only five months. Chandra has resolved most of the X-ray background, a pervasive glow of X-rays throughout the universe, first discovered in the early days of space exploration. Before now, scientists have not been able to discern the background's origin, because no X-ray telescope until Chandra has had both the angular resolution and sensitivity to resolve it. "This is a major discovery," said Dr. Alan Bunner, Director of NASA's Structure andEvolution of the universe science theme. "Since it was first observed thirty-seven years ago, understanding the source of the X-ray background has been aHoly Grail of X-ray astronomy. Now, it is within reach." The results of the observation will be discussed today at the 195th national meeting of the American Astronomical Society in Atlanta, Georgia. An article describing this work has been submitted to the journal Nature by Dr. Richard Mushotzky, of NASA Goddard Space Flight Center, Greenbelt, Md., Drs. Lennox Cowie and Amy Barger at the University of Hawaii, Honolulu, and Dr. Keith Arnaud of the University of Maryland, College Park. "We are all very excited by this finding," said Mushotzky. "The resolution of most of the hard X-ray background during the first few months of the Chandra mission is a tribute to the power of this observatory and bodes extremely well for its scientific future," Scientists have known about the X-ray glow, called the X-ray background, since the dawn of X-ray astronomy in the early 1960s. They have been unable to discern its origin, however, for no X-ray telescope until Chandra has had both the angular resolution and sensitivity to resolve it. The German-led ROSAT mission, now completed, resolved much of the lower

  20. X-ray optical diagnostic of laser produced plasmas for nuclear fusion and X-ray lasers

    Energy Technology Data Exchange (ETDEWEB)

    Butzbach, R.

    2001-07-01

    In the present work, the conception, design and appliance of toroidally bent crystals for the X-ray optical diagnostics of laser produced plasmas is discussed. The first part of this work deals with the development, design and characterization of an X-Ray microscope for the observation of Rayleigh-Taylor instabilities, which act against the confinement and ignition of the fuel in the inertial confinement fusion process. The aim of the second part of the present work was the diagnostic of the lasing medium for amplified spontaneous emission close to the water window. For this purpose, an one-dimensionally (1-D) imaging X-ray spectrometer based on toroidally bent quartz crystals was developed for the observation of the Ni-like 4f-3d transition of Yb, Hf, Ta, and W ions, which should be related to the amplified 4d-4p emission, since the 4f niveau is very close to the 4d niveau. Thus, the 4f-3d transition can serve as an indicator for the population of the 4d niveau. (orig.)

  1. Nonlocal heat transport and improved target design for x-ray heating studies at x-ray free electron lasers

    Science.gov (United States)

    Hoidn, Oliver; Seidler, Gerald T.

    2018-01-01

    The extremely high-power densities and short durations of single pulses of x-ray free electron lasers (XFELs) have opened new opportunities in atomic physics, where complex excitation-relaxation chains allow for high ionization states in atomic and molecular systems, and in dense plasma physics, where XFEL heating of solid-density targets can create unique dense states of matter having temperatures on the order of the Fermi energy. We focus here on the latter phenomena, with special emphasis on the problem of optimum target design to achieve high x-ray heating into the warm dense matter (WDM) state. We report fully three-dimensional simulations of the incident x-ray pulse and the resulting multielectron relaxation cascade to model the spatial energy density deposition in multicomponent targets, with particular focus on the effects of nonlocal heat transport due to the motion of high energy photoelectrons and Auger electrons. We find that nanoscale high-Z /low-Z multicomponent targets can give much improved energy density deposition in lower-Z materials, with enhancements reaching a factor of 100. This has three important benefits. First, it greatly enlarges the thermodynamic parameter space in XFEL x-ray heating studies of lower-Z materials. Second, it allows the use of higher probe photon energies, enabling higher-information content x-ray diffraction (XRD) measurements such as in two-color XFEL operations. Third, while this is merely one step toward optimization of x-ray heating target design, the demonstration of the importance of nonlocal heat transport establishes important common ground between XFEL-based x-ray heating studies and more traditional laser plasma methods.

  2. Development of laser plasma x-ray microscope for living hydrated biological specimens

    International Nuclear Information System (INIS)

    Kado, Masataka; Daido, Hiroyuki

    2005-01-01

    Investigating the structure and the function of life object performing advanced life activity becomes important. In order to investigate the life object, it is necessary to observe living specimens with high spatial resolution and high temporal resolution. Since laser plasma x-ray source has high brightness and short pulse duration, x-ray microscope with the laser plasma x-ray source makes possible to observe living specimens. Such as chromosomes, macrophages, bacterium, and so on have been observed by contact x-ray microscopy. The x-ray images obtained by indirect measurements such as the contact x-ray microscopy have difficulty to avoid artificial effect such as irregular due to developing process. Development of an x-ray microscope with laser plasma x-ray source is necessary to avoid such defects. (author)

  3. Compton polarimetry with position-resolving X-ray detectors

    International Nuclear Information System (INIS)

    Hess, Sebastian

    2010-02-01

    In the present thesis the prototype of a novel position-resolving and multi-hit able 2D Si(Li) strip detector is characterized, the planar detector crystal of which is simultaneously applied both as scatterer and as absorber. In the framework of this thesis the Si(Li) polarimeter could be applied in different experiments on the radiative electron capture and on the characteristic radiation at the experimental storage ring of the GSI. The characterization of the detector pursued by means of the highly polarized radiation of the electron capture into the K shell of naked xenon. In the following in two further experiments new values on the polarization of the electron capture into the K shell both of the naked and of the hydrogen-like uranium were performed.

  4. RESOLVED COMPANIONS OF CEPHEIDS: TESTING THE CANDIDATES WITH X-RAY OBSERVATIONS

    Energy Technology Data Exchange (ETDEWEB)

    Evans, Nancy Remage; Pillitteri, Ignazio; Wolk, Scott; Karovska, Margarita; Tingle, Evan [Smithsonian Astrophysical Observatory, MS 4, 60 Garden St., Cambridge, MA 02138 (United States); Guinan, Edward; Engle, Scott [Department of Astronomy and Astrophysics, Villanova University, 800 Lancaster Ave., Villanova, PA 19085 (United States); Bond, Howard E. [Department of Astronomy and Astrophysics, Pennsylvania State University, University Park, PA 16802 (United States); Schaefer, Gail H. [The CHARA Array of Georgia State University, Mount Wilson, California 91023 (United States); Mason, Brian D., E-mail: nevans@cfa.harvard.edu, E-mail: heb11@psu.edu, E-mail: schaefer@chara-array.org [US Naval Observatory, 3450 Massachusetts Ave., NW, Washington, DC 20392-5420 (United States)

    2016-04-15

    We have made XMM-Newton observations of 14 Galactic Cepheids that have candidate resolved (≥5″) companion stars based on our earlier HST Wide Field Camera 3 (WFC3) imaging survey. Main-sequence stars that are young enough to be physical companions of Cepheids are expected to be strong X-ray producers in contrast to field stars. XMM-Newton exposures were set to detect essentially all companions hotter than spectral type M0 (corresponding to 0.5 M{sub ⊙}). The large majority of our candidate companions were not detected in X-rays, and hence are not confirmed as young companions. One resolved candidate (S Nor #4) was unambiguously detected, but the Cepheid is a member of a populous cluster. For this reason, it is likely that S Nor #4 is a cluster member rather than a gravitationally bound companion. Two further Cepheids (S Mus and R Cru) have X-ray emission that might be produced by either the Cepheid or the candidate resolved companion. A subsequent Chandra observation of S Mus shows that the X-rays are at the location of the Cepheid/spectroscopic binary. R Cru and also V659 Cen (also X-ray bright) have possible companions closer than 5″ (the limit for this study) which are the likely sources of X-rays. One final X-ray detection (V473 Lyr) has no known optical companion, so the prime suspect is the Cepheid itself. It is a unique Cepheid with a variable amplitude. The 14 stars that we observed with XMM constitute 36% of the 39 Cepheids found to have candidate companions in our HST/WFC3 optical survey. No young probable binary companions were found with separations of ≥5″ or 4000 au.

  5. RESOLVED COMPANIONS OF CEPHEIDS: TESTING THE CANDIDATES WITH X-RAY OBSERVATIONS

    International Nuclear Information System (INIS)

    Evans, Nancy Remage; Pillitteri, Ignazio; Wolk, Scott; Karovska, Margarita; Tingle, Evan; Guinan, Edward; Engle, Scott; Bond, Howard E.; Schaefer, Gail H.; Mason, Brian D.

    2016-01-01

    We have made XMM-Newton observations of 14 Galactic Cepheids that have candidate resolved (≥5″) companion stars based on our earlier HST Wide Field Camera 3 (WFC3) imaging survey. Main-sequence stars that are young enough to be physical companions of Cepheids are expected to be strong X-ray producers in contrast to field stars. XMM-Newton exposures were set to detect essentially all companions hotter than spectral type M0 (corresponding to 0.5 M ⊙ ). The large majority of our candidate companions were not detected in X-rays, and hence are not confirmed as young companions. One resolved candidate (S Nor #4) was unambiguously detected, but the Cepheid is a member of a populous cluster. For this reason, it is likely that S Nor #4 is a cluster member rather than a gravitationally bound companion. Two further Cepheids (S Mus and R Cru) have X-ray emission that might be produced by either the Cepheid or the candidate resolved companion. A subsequent Chandra observation of S Mus shows that the X-rays are at the location of the Cepheid/spectroscopic binary. R Cru and also V659 Cen (also X-ray bright) have possible companions closer than 5″ (the limit for this study) which are the likely sources of X-rays. One final X-ray detection (V473 Lyr) has no known optical companion, so the prime suspect is the Cepheid itself. It is a unique Cepheid with a variable amplitude. The 14 stars that we observed with XMM constitute 36% of the 39 Cepheids found to have candidate companions in our HST/WFC3 optical survey. No young probable binary companions were found with separations of ≥5″ or 4000 au

  6. Resolved Companions of Cepheids: Testing the Candidates with X-Ray Observations

    Science.gov (United States)

    Evans, Nancy Remage; Pillitteri, Ignazio; Wolk, Scott; Karovska, Margarita; Tingle, Evan; Guinan, Edward; Engle, Scott; Bond, Howard E.; Schaefer, Gail H.; Mason, Brian D.

    2016-04-01

    We have made XMM-Newton observations of 14 Galactic Cepheids that have candidate resolved (≥5″) companion stars based on our earlier HST Wide Field Camera 3 (WFC3) imaging survey. Main-sequence stars that are young enough to be physical companions of Cepheids are expected to be strong X-ray producers in contrast to field stars. XMM-Newton exposures were set to detect essentially all companions hotter than spectral type M0 (corresponding to 0.5 M⊙). The large majority of our candidate companions were not detected in X-rays, and hence are not confirmed as young companions. One resolved candidate (S Nor #4) was unambiguously detected, but the Cepheid is a member of a populous cluster. For this reason, it is likely that S Nor #4 is a cluster member rather than a gravitationally bound companion. Two further Cepheids (S Mus and R Cru) have X-ray emission that might be produced by either the Cepheid or the candidate resolved companion. A subsequent Chandra observation of S Mus shows that the X-rays are at the location of the Cepheid/spectroscopic binary. R Cru and also V659 Cen (also X-ray bright) have possible companions closer than 5″ (the limit for this study) which are the likely sources of X-rays. One final X-ray detection (V473 Lyr) has no known optical companion, so the prime suspect is the Cepheid itself. It is a unique Cepheid with a variable amplitude. The 14 stars that we observed with XMM constitute 36% of the 39 Cepheids found to have candidate companions in our HST/WFC3 optical survey. No young probable binary companions were found with separations of ≥5″ or 4000 au. Based on observations obtained with XMM-Newton, an ESA science mission with instruments and contributions directly funded by ESA Member States and the USA (NASA).

  7. Simulation of intense laser-dense matter interactions. X-ray production and laser absorption

    Energy Technology Data Exchange (ETDEWEB)

    Ueshima, Yutaka; Kishimoto, Yasuaki; Sasaki, Akira [Japan Atomic Energy Research Inst., Neyagawa, Osaka (Japan). Kansai Research Establishment; Sentoku, Yasuhiko; Tajima, Toshiki

    1998-03-01

    The development of short-pulse ultra high intensity lasers will enable us to generate short-pulse intense soft and hard X-rays. Acceleration of an electron in laser field generates intense illuminated located radiation, Larmor radiation, around KeV at 10{sup 18} W/cm{sup 2} with 100 TW and 1 {mu}m wave length laser. The Coulomb interaction between rest ions and relativistic electron generates broad energy radiation, bremsstrahlung emission, over MeV at 10{sup 18} W/cm{sup 2} with the same condition. These intense radiations come in short pulses of the same order as that of the irradiated laser. The generated intense X-rays, Larmor and bremsstrahlung radiation, can be applied to sources of short pulse X-ray, excitation source of inner-shell X-ray laser, position production and nuclear excitation, etc. (author)

  8. Development of x-ray laser architectural components

    International Nuclear Information System (INIS)

    Wan, A.S.; Da Silva, L.B.; Moreno, J.C.

    1994-06-01

    This paper describes the recent experimental and computational development of short-pulse, enhanced-coherence, and high-brilliance x-ray lasers (XRLs). The authors will describe the development of an XRL cavity by injecting laser photons back into an amplifying XRL plasma. Using a combination of LASNEX/GLF/SPECTRE-BEAM3 codes, they obtained good agreement with experimental results. They will describe the adaptive spatial filtering technique used to design small-aperture shaped XRLs with near diffraction-limited output. Finally they will discuss issues concerning the development of high-brilliance XRL architecture, with emphasis on scaling the XRL aperture. Combining these advances in XRL architectural components allows them to develop a short-pulse, high-brilliance, coherent XRL suitable for applications in areas such as biological holography, plasma interferometry, and nonlinear optics

  9. High efficiency, multiterawatt x-ray free electron lasers

    Directory of Open Access Journals (Sweden)

    C. Emma

    2016-02-01

    Full Text Available In this paper we present undulator magnet tapering methods for obtaining high efficiency and multiterawatt peak powers in x-ray free electron lasers (XFELs, a key requirement for enabling 3D atomic resolution single molecule imaging and nonlinear x-ray science. The peak power and efficiency of tapered XFELs is sensitive to time dependent effects, like synchrotron sideband growth. To analyze this dependence in detail we perform a comparative numerical optimization for the undulator magnetic field tapering profile including and intentionally disabling these effects. We show that the solution for the magnetic field taper profile obtained from time independent optimization does not yield the highest extraction efficiency when time dependent effects are included. Our comparative optimization is performed for a novel undulator designed specifically to obtain TW power x-ray pulses in the shortest distance: superconducting, helical, with short period and built-in strong focusing. This design reduces the length of the breaks between modules, decreasing diffraction effects, and allows using a stronger transverse electron focusing. Both effects reduce the gain length and the overall undulator length. We determine that after a fully time dependent optimization of a 100 m long Linac coherent light source-like XFEL we can obtain a maximum efficiency of 7%, corresponding to 3.7 TW peak radiation power. Possible methods to suppress the synchrotron sidebands, and further enhance the FEL peak power, up to about 6 TW by increasing the seed power and reducing the electron beam energy spread, are also discussed.

  10. A comparative study of the ionic keV X-ray line emission from ...

    Indian Academy of Sciences (India)

    resolved X-ray diffraction [15] etc. High conversion efficiency of the laser ... picosecond ionic X-ray pulses are produced when both the plasma density and the tem- ..... X-ray spectrum of magnesium plasma produced using femtosecond laser.

  11. Visible/IR light and x-rays in femtosecond synchronism from an x-ray free-electron laser

    International Nuclear Information System (INIS)

    Adams, B. A.; Experimental Facilities Division

    2005-01-01

    A way is proposed to obtain pulses of visible/infrared light in femtosecond synchronism with x-rays from an x-ray free-electron laser (XFEL), using the recently proposed emittance-slicing technique. In an XFEL undulator, only the short section of an electron bunch whose emittance is left unchanged by the slicing will emit intense coherent x-rays in the XFEL undulator. At the same time, the bunch emits highly collimated transition undulator radiation (TUR) into a cone whose opening angle is the reciprocal relativisticity parameter gamma. Due to the variation of the transverse momentum induced by the emittance slicing, the effective number of charges contributing to the TUR varies along the bunch, and is higher in the sliced-out part that emits the coherent x-rays. As with coherent synchrotron radiation (CSR), the TUR is thus coherently enhanced (CTUR) at near-infrared wavelengths. Coming from the same part of the bunch the CTUR and the coherent x-rays are perfectly synchronized to each other. Because both types of radiation are generated in the long straight XFEL undulator, there are no dispersion effects that might induce a timing jitter. With typical XFEL parameters, the energy content of the single optical cycle of near-IR CTUR light is about 100 Nano-Joule, which is quite sufficient for most pump-probe experiments

  12. Laser micromachining of cadmium tungstate scintillator for high energy X-ray imaging

    Science.gov (United States)

    Richards, Sion Andreas

    Pulsed laser ablation has been investigated as a method for the creation of thick segmented scintillator arrays for high-energy X-ray radiography. Thick scintillators are needed to improve the X-ray absorption at high energies, while segmentation is required for spatial resolution. Monte-Carlo simulations predicted that reflections at the inter-segment walls were the greatest source of loss of scintillation photons. As a result of this, fine pitched arrays would be inefficient as the number of reflections would be significantly higher than in large pitch arrays. Nanosecond and femtosecond pulsed laser ablation was investigated as a method to segment cadmium tungstate (CdWO_4). The effect of laser parameters on the ablation mechanisms, laser induced material changes and debris produced were investigated using optical and electron microscopy, energy dispersive X-ray spectroscopy and X-ray photoelectron spectroscopy for both types of lasers. It was determined that nanosecond ablation was unsuitable due to the large amount of cracking and a heat affected zone created during the ablation process. Femtosecond pulsed laser ablation was found to induce less damage. The optimised laser parameters for a 1028 nm laser was found to be a pulse energy of 54 μJ corresponding to a fluence of 5.3 J cm. -2 a pulse duration of 190 fs, a repetition rate of 78.3 kHz and a laser scan speed of 707 mm s. -1 achieving a normalised pulse overlap of 0.8. A serpentine scan pattern was found to minimise damage caused by anisotropic thermal expansion. Femtosecond pulsed ablation was also found to create a layer of tungsten and cadmium sub-oxides on the surface of the crystals. The CdWO_4 could be cleaned by immersing the CdWO_4 in ammonium hydroxide at 45°C for 15 minutes. However, XPS indicated that the ammonium hydroxide formed a thin layer of CdCO_3 and Cd(OH)_2 on the surface. Prototype arrays were shown to be able to resolve features as small as 0.5 mm using keV energy X-rays. The most

  13. Determining grain resolved stresses in polycrystalline materials using three-dimensional X-ray diffraction

    DEFF Research Database (Denmark)

    Oddershede, Jette; Schmidt, Søren; Poulsen, Henning Friis

    2010-01-01

    An algorithm is presented for characterization of the grain resolved (type II) stress states in a polycrystalline sample based on monochromatic X-ray diffraction data. The algorithm is a robust 12-parameter-per-grain fit of the centre-of-mass grain positions, orientations and stress tensors...

  14. Reflection of attosecond x-ray free electron laser pulses

    International Nuclear Information System (INIS)

    Hau-Riege, Stefan P.; Chapman, Henry N.

    2007-01-01

    In order to utilize hard x-ray free electron lasers (XFEL's) when they are extended to attosecond pulse lengths, it is necessary to choose optical elements with minimal response time. Specular grazing-incidence optics made of low-Z materials are popular candidates for reflectors since they are likely to withstand x-ray damage and provide sufficiently large reflectivities. Using linear-optics reflection theory, we calculated the transient reflectivity of a delta-function electric pulse from a homogenous semi-infinite medium as a function of angle of incidence for s- and p-polarized light. We specifically considered the pulse response of beryllium, diamond, silicon carbide, and silicon, all of which are of relevance to the XFEL's that are currently being built. We found that the media emit energy in a damped oscillatory way, and that the impulse-response times are shorter than 0.3 fs for normal incidence. For grazing incidence, the impulse-response time is substantially shorter, making grazing-incidence mirrors a good choice for deep subfemtosecond reflective optics

  15. Time-resolved and position-resolved X-ray spectrometry with a pixelated detector

    Energy Technology Data Exchange (ETDEWEB)

    Sievers, Peter

    2012-12-07

    show a good agreement. Up to now the measurements of impinging spectra with a Timepix detector have been performed in radiation fields with a relatively high fluence. To cope with the requirement of measuring in radiation fields with a low fluence, there had to be changes in the method of analysis compared to those performed formerly. An important improvement in this context was the employment of the Bayesian deconvolution method. The spectra reconstructed with this method were then compared to the results of two different and established detection systems. Firstly, the shape of the deconvolved spectrum was compared to the one measured with a hpGe detector. Secondly, the calculated value of the kerma rate was compared to the one measured with an ionization chamber. This gave an estimate on the correctness of the absolute number of photons. Both comparisons have shown a good agreement and thus I was able to validate that the method delivers precise results. Compared to the formerly used spectrum-stripping method the Bayesian deconvolution turned out to be very stable and reliable. This robustness of the deconvolution method and the development of a pixel-by-pixel energy calibration were the keys towards position-resolved spectrometry. With such a precise energy calibration the energy resolution was enhanced by up to 45%. This improved accuracy in the measurement has been very demanding on the improvements of the simulation of the response matrix needed for deconvolution. Both this enhanced simulation and a pixel-by-pixel calibrated detector opened the possibility of measuring the anode heel effect. Not only the relative angular dependency of the spectrum emitted but also the change in the absolute photon fluence were measured. Furthermore, it is possible to even use small ROIs down to 4x4 pixels to evaluate a spectrum. This was then applied for the spectrometry of small focal spots of a miniature X-ray source used in therapeutics. Furthermore, the robustness and the

  16. Time-resolved and position-resolved X-ray spectrometry with a pixelated detector

    International Nuclear Information System (INIS)

    Sievers, Peter

    2012-01-01

    show a good agreement. Up to now the measurements of impinging spectra with a Timepix detector have been performed in radiation fields with a relatively high fluence. To cope with the requirement of measuring in radiation fields with a low fluence, there had to be changes in the method of analysis compared to those performed formerly. An important improvement in this context was the employment of the Bayesian deconvolution method. The spectra reconstructed with this method were then compared to the results of two different and established detection systems. Firstly, the shape of the deconvolved spectrum was compared to the one measured with a hpGe detector. Secondly, the calculated value of the kerma rate was compared to the one measured with an ionization chamber. This gave an estimate on the correctness of the absolute number of photons. Both comparisons have shown a good agreement and thus I was able to validate that the method delivers precise results. Compared to the formerly used spectrum-stripping method the Bayesian deconvolution turned out to be very stable and reliable. This robustness of the deconvolution method and the development of a pixel-by-pixel energy calibration were the keys towards position-resolved spectrometry. With such a precise energy calibration the energy resolution was enhanced by up to 45%. This improved accuracy in the measurement has been very demanding on the improvements of the simulation of the response matrix needed for deconvolution. Both this enhanced simulation and a pixel-by-pixel calibrated detector opened the possibility of measuring the anode heel effect. Not only the relative angular dependency of the spectrum emitted but also the change in the absolute photon fluence were measured. Furthermore, it is possible to even use small ROIs down to 4x4 pixels to evaluate a spectrum. This was then applied for the spectrometry of small focal spots of a miniature X-ray source used in therapeutics. Furthermore, the robustness and the

  17. Measurement of the spatial coherence of a soft x-ray laser

    International Nuclear Information System (INIS)

    Trebes, J.E.; Mrowka, S.; London, R.A.; Barbee, T.W.; Carter, M.R.; MacGowan, B.J.; Matthews, D.L.; Da Silva, L.B.; Stone, G.F.; Feit, M.D.; Nugent, K.A.

    1991-01-01

    The spatial coherence of a neon-like selenium x-ray laser operating at 206 and 210 Angstroems has been measured using a technique based on partially coherent x-ray diffraction. The time integrated spatial coherence of the selenium x-ray laser was determined to be equivalent to that of a quasi-monochromatic spatially incoherent disk source whose diameter is comparable to the line focus of the visible light laser pumping the x-ray laser. The spatial coherence was improved by narrowing the line focus width. 20 refs., 4 figs

  18. X-ray diagnostics in the laser-initiated fusion program

    International Nuclear Information System (INIS)

    Godwin, R.P.

    1975-08-01

    The high-density and high-temperature plasma conditions required for successful laser-initiated fusion make x-ray diagnostics a valuable tool in this exciting field. Measurements of the hard x-ray continuum emitted from laser targets provide insight into the complex laser-plasma coupling physics and the consequent energy transport through the bremsstrahlung signature of energetic electrons. X-ray techniques are important in the selection and assay of microballoon targets for current compression experiments. X-ray imaging experiments and diffraction spectroscopy of highly stripped atoms can provide information upon the symmetry, density and temperature of laser targets. Extremely high temporal and spatial resolution may be required for definitive diagnostic information on compressed targets. While laser-produced plasmas are interesting as possible intense x-ray sources and as a possible means of achieving x-ray lasing, those topics are outside the scope of this review. (auth)

  19. Development and characterization of femtosecond laser driven soft x-ray lasers

    International Nuclear Information System (INIS)

    Bettaibi, I.

    2005-06-01

    Coherent soft x-ray sources have an important potential for scientific, medical and industrial applications. The development of high intensity laser systems allowed the realization of new coherent and fast soft x-ray sources like high order harmonic generation and soft x-ray lasers. These sources are compact, cheaper than traditional sources such as synchrotrons, and are thus interesting. This thesis presents the study of a new soft x-ray laser pumped by a femto-second laser beam working at 10 Hz. The circularly polarized ultra intense laser is longitudinally focused in a cell filled with xenon or krypton, to obtain the amplification of two lasing lines at 41.8 nm and 32.8 nm in Pd-like xenon and Ni-like krypton respectively. We carry out an experimental and numerical study of the source to understand the importance of different parameters such as the laser intensity and polarization, the gas pressure and the cell length. We have also spatially and temporally characterized the soft x-ray laser beam. To compensate the refraction of the driving laser we have investigated guiding techniques consisting in creating a plasma channel by electric discharge or using the multiple reflections of the driving laser on the internal walls of the dielectric tubes of sapphire or glass. A spectacular improvement of the source performances has been observed in both cases. Finally, we present a preliminary study on a different x-ray scheme: the inner shell photo pumping of neutral atoms. We have developed an optical system, which should create the appropriate conditions for the realisation of short wavelength x-ray amplifier. (author)

  20. Element-resolved x-ray ferrimagnetic and ferromagnetic resonance spectroscopy

    International Nuclear Information System (INIS)

    Boero, G; Mouaziz, S; Rusponi, S; Bencok, P; Nolting, F; Stepanow, S; Gambardella, P

    2008-01-01

    We report on the measurement of element-specific magnetic resonance spectra at gigahertz frequencies using x-ray magnetic circular dichroism (XMCD). We investigate the ferrimagnetic precession of Gd and Fe ions in Gd-substituted yttrium iron garnet, showing that the resonant field and linewidth of Gd precisely coincide with Fe up to the nonlinear regime of parametric excitations. The opposite sign of the Gd x-ray magnetic resonance signal with respect to Fe is consistent with dynamic antiferromagnetic alignment of the two ionic species. Further, we investigate a bilayer metal film, Ni 80 Fe 20 (5 nm)/Ni(50 nm), where the coupled resonance modes of Ni and Ni 80 Fe 20 are separately resolved, revealing shifts in the resonance fields of individual layers but no mutual driving effects. Energy-dependent dynamic XMCD measurements are introduced, combining x-ray absorption and magnetic resonance spectroscopies

  1. Multi-scale mechanics of granular solids from grain-resolved X-ray measurements

    Science.gov (United States)

    Hurley, R. C.; Hall, S. A.; Wright, J. P.

    2017-11-01

    This work discusses an experimental technique for studying the mechanics of three-dimensional (3D) granular solids. The approach combines 3D X-ray diffraction and X-ray computed tomography to measure grain-resolved strains, kinematics and contact fabric in the bulk of a granular solid, from which continuum strains, grain stresses, interparticle forces and coarse-grained elasto-plastic moduli can be determined. We demonstrate the experimental approach and analysis of selected results on a sample of 1099 stiff, frictional grains undergoing multiple uniaxial compression cycles. We investigate the inter-particle force network, elasto-plastic moduli and associated length scales, reversibility of mechanical responses during cyclic loading, the statistics of microscopic responses and microstructure-property relationships. This work serves to highlight both the fundamental insight into granular mechanics that is furnished by combined X-ray measurements and describes future directions in the field of granular materials that can be pursued with such approaches.

  2. Resolving hot spot microstructure using x-ray penumbral imaging (invited)

    Science.gov (United States)

    Bachmann, B.; Hilsabeck, T.; Field, J.; Masters, N.; Reed, C.; Pardini, T.; Rygg, J. R.; Alexander, N.; Benedetti, L. R.; Döppner, T.; Forsman, A.; Izumi, N.; LePape, S.; Ma, T.; MacPhee, A. G.; Nagel, S.; Patel, P.; Spears, B.; Landen, O. L.

    2016-11-01

    We have developed and fielded x-ray penumbral imaging on the National Ignition Facility in order to enable sub-10 μm resolution imaging of stagnated plasma cores (hot spots) of spherically shock compressed spheres and shell implosion targets. By utilizing circular tungsten and tantalum apertures with diameters ranging from 20 μm to 2 mm, in combination with image plate and gated x-ray detectors as well as imaging magnifications ranging from 4 to 64, we have demonstrated high-resolution imaging of hot spot plasmas at x-ray energies above 5 keV. Here we give an overview of the experimental design criteria involved and demonstrate the most relevant influences on the reconstruction of x-ray penumbral images, as well as mitigation strategies of image degrading effects like over-exposed pixels, artifacts, and photon limited source emission. We describe experimental results showing the advantages of x-ray penumbral imaging over conventional Fraunhofer and photon limited pinhole imaging and showcase how internal hot spot microstructures can be resolved.

  3. Resolving hot spot microstructure using x-ray penumbral imaging (invited)

    Energy Technology Data Exchange (ETDEWEB)

    Bachmann, B., E-mail: bachmann2@llnl.gov; Field, J.; Masters, N.; Pardini, T.; Rygg, J. R.; Benedetti, L. R.; Döppner, T.; Izumi, N.; LePape, S.; Ma, T.; MacPhee, A. G.; Nagel, S.; Patel, P.; Spears, B.; Landen, O. L. [Lawrence Livermore National Laboratory, Livermore, California 94550 (United States); Hilsabeck, T.; Reed, C.; Alexander, N.; Forsman, A. [General Atomics, San Diego, California 92186 (United States)

    2016-11-15

    We have developed and fielded x-ray penumbral imaging on the National Ignition Facility in order to enable sub-10 μm resolution imaging of stagnated plasma cores (hot spots) of spherically shock compressed spheres and shell implosion targets. By utilizing circular tungsten and tantalum apertures with diameters ranging from 20 μm to 2 mm, in combination with image plate and gated x-ray detectors as well as imaging magnifications ranging from 4 to 64, we have demonstrated high-resolution imaging of hot spot plasmas at x-ray energies above 5 keV. Here we give an overview of the experimental design criteria involved and demonstrate the most relevant influences on the reconstruction of x-ray penumbral images, as well as mitigation strategies of image degrading effects like over-exposed pixels, artifacts, and photon limited source emission. We describe experimental results showing the advantages of x-ray penumbral imaging over conventional Fraunhofer and photon limited pinhole imaging and showcase how internal hot spot microstructures can be resolved.

  4. Versatile, reprogrammable area pixel array detector for time-resolved synchrotron x-ray applications

    Energy Technology Data Exchange (ETDEWEB)

    Gruner, Sol [Cornell Univ., Ithaca, NY (United States)

    2010-05-01

    The final technical report for DOE grant DE-SC0004079 is presented. The goal of the grant was to perform research, development and application of novel imaging x-ray detectors so as to effectively utilize the high intensity and brightness of the national synchrotron radiation facilities to enable previously unfeasible time-resolved x-ray research. The report summarizes the development of the resultant imaging x-ray detectors. Two types of detector platforms were developed: The first is a detector platform (called a Mixed-Mode Pixel Array Detector, or MM-PAD) that can image continuously at over a thousand images per second while maintaining high efficiency for wide dynamic range signals ranging from 1 to hundreds of millions of x-rays per pixel per image. Research on an even higher dynamic range variant is also described. The second detector platform (called the Keck Pixel Array Detector) is capable of acquiring a burst of x-ray images at a rate of millions of images per second.

  5. Resolving hot spot microstructure using x-ray penumbral imaging (invited).

    Science.gov (United States)

    Bachmann, B; Hilsabeck, T; Field, J; Masters, N; Reed, C; Pardini, T; Rygg, J R; Alexander, N; Benedetti, L R; Döppner, T; Forsman, A; Izumi, N; LePape, S; Ma, T; MacPhee, A G; Nagel, S; Patel, P; Spears, B; Landen, O L

    2016-11-01

    We have developed and fielded x-ray penumbral imaging on the National Ignition Facility in order to enable sub-10 μm resolution imaging of stagnated plasma cores (hot spots) of spherically shock compressed spheres and shell implosion targets. By utilizing circular tungsten and tantalum apertures with diameters ranging from 20 μm to 2 mm, in combination with image plate and gated x-ray detectors as well as imaging magnifications ranging from 4 to 64, we have demonstrated high-resolution imaging of hot spot plasmas at x-ray energies above 5 keV. Here we give an overview of the experimental design criteria involved and demonstrate the most relevant influences on the reconstruction of x-ray penumbral images, as well as mitigation strategies of image degrading effects like over-exposed pixels, artifacts, and photon limited source emission. We describe experimental results showing the advantages of x-ray penumbral imaging over conventional Fraunhofer and photon limited pinhole imaging and showcase how internal hot spot microstructures can be resolved.

  6. Resolving hot spot microstructure using x-ray penumbral imaging (invited)

    International Nuclear Information System (INIS)

    Bachmann, B.; Field, J.; Masters, N.; Pardini, T.; Rygg, J. R.; Benedetti, L. R.; Döppner, T.; Izumi, N.; LePape, S.; Ma, T.; MacPhee, A. G.; Nagel, S.; Patel, P.; Spears, B.; Landen, O. L.; Hilsabeck, T.; Reed, C.; Alexander, N.; Forsman, A.

    2016-01-01

    We have developed and fielded x-ray penumbral imaging on the National Ignition Facility in order to enable sub-10 μm resolution imaging of stagnated plasma cores (hot spots) of spherically shock compressed spheres and shell implosion targets. By utilizing circular tungsten and tantalum apertures with diameters ranging from 20 μm to 2 mm, in combination with image plate and gated x-ray detectors as well as imaging magnifications ranging from 4 to 64, we have demonstrated high-resolution imaging of hot spot plasmas at x-ray energies above 5 keV. Here we give an overview of the experimental design criteria involved and demonstrate the most relevant influences on the reconstruction of x-ray penumbral images, as well as mitigation strategies of image degrading effects like over-exposed pixels, artifacts, and photon limited source emission. We describe experimental results showing the advantages of x-ray penumbral imaging over conventional Fraunhofer and photon limited pinhole imaging and showcase how internal hot spot microstructures can be resolved.

  7. Streaked spectrometry using multilayer x-ray-interference mirrors to investigate energy transport in laser-plasma applications

    International Nuclear Information System (INIS)

    Stradling, G.L.; Barbee, T.W. Jr.; Henke, B.L.; Campbell, E.M.; Mead, W.C.

    1981-08-01

    Transport of energy in laser-produced plasmas is scrutinized by devising spectrally and temporally identifiable characteristics in the x-ray emission history which identify the heat-front position at various times in the heating process. Measurements of the relative turn-on times of these characteristics show the rate of energy transport between various points. These measurements can in turn constrain models of energy transport phenomena. We are time-resolving spectrally distinguishable subkilovolt x-ray emissions from different layers of a disk target to examine the transport rate of energy into the target. A similar technique is used to measure the lateral expansion rate of the plasma spot. A soft x-ray streak camera with 15-psec temporal resolution is used to make the temporal measurements. Spectral discrimination of the incident signal is provided by multilayer x-ray interference mirrors

  8. Platform development of x-ray absorption-based temperature measurements above 100-eV on the OMEGA laser

    Science.gov (United States)

    Workman, Jonathan; Keiter, P.; Tierney, T.; Tierney, H.; Belle, K.; Magelssen, G.; Peterson, R.; Fryer, C.; Comley, A.; Taylor, M.

    2007-11-01

    Experiments were performed on the OMEGA laser system at the University of Rochester to measure radiation temperature in hohlraum-heated foams. Using x-ray absorption spectroscopy in the 3-6-keV x-ray range allows temperature determination in the range of 50-200-eV. Uranium, bismuth and gold M-shell x-ray emission were used as broadband backlighters. Backlighter absorption through heated chlorinated foam and scandium tracers were used to determine temperatures. The development of this technique in the temperature range of 100-200-eV will be used for platform development of future NIF experiments. We will present time-integrated and time-resolved measurements of x-ray emission from the backlighter materials as well as absorption measurements trough the heated tracer materials. We will also present future directions in the development of this platform.

  9. Photolysis of Br2 in CCl4 studied by time-resolved X-ray scattering.

    Science.gov (United States)

    Kong, Qingyu; Lee, Jae Hyuk; Lo Russo, Manuela; Kim, Tae Kyu; Lorenc, Maciej; Cammarata, Marco; Bratos, Savo; Buslaps, Thomas; Honkimaki, Veijo; Ihee, Hyotcherl; Wulff, Michael

    2010-03-01

    A time-resolved X-ray solution scattering study of bromine molecules in CCl(4) is presented as an example of how to track atomic motions in a simple chemical reaction. The structures of the photoproducts are tracked during the recombination process, geminate and non-geminate, from 100 ps to 10 micros after dissociation. The relaxation of hot Br(2)(*) molecules heats the solvent. At early times, from 0.1 to 10 ns, an adiabatic temperature rise is observed, which leads to a pressure gradient that forces the sample to expand. The expansion starts after about 10 ns with the laser beam sizes used here. When thermal artefacts are removed by suitable scaling of the transient solvent response, the excited-state solute structures can be obtained with high fidelity. The analysis shows that 30% of Br(2)(*) molecules recombine directly along the X potential, 60% are trapped in the A/A' state with a lifetime of 5.5 ns, and 10% recombine non-geminately via diffusive motion in about 25 ns. The Br-Br distance distribution in the A/A' state peaks at 3.0 A.

  10. Dynamics of a multiple-pulse-driven x-ray laser plasma

    International Nuclear Information System (INIS)

    Wan, A.S.; Da Silva, L.B.; Moreno, J.C.; Cauble, R.; Celliers, P.; Dalhed, H.E. Jr.; Koch, J.A.; Nilsen, J.

    1996-01-01

    In this paper we describe experimental and computational studies of multiple-pulse-driven laser plasma, which is the gain medium for a neon-like yttrium x-ray laser. Near-field emission profiles have been measured both with and without reinjection of the x-ray laser photons to couple with the amplifying medium created by later pulses using an external multilayer mirror. From the temporal and spatial evolution of the near-field emission profiles we can examine the pulse-to-pulse variation of the x-ray laser plasma due to changes in the hydrodynamics, laser deposition, and the injecting of x-ray laser photons back into an amplifying x-ray laser plasma. Using a combination of radiation hydrodynamics, atomic kinetics, and ray propagation codes, reasonable agreement has been obtained between simulations and the experimental results. copyright 1996 American Institute of Physics

  11. X-ray absorption spectroscopy using a self-seeded soft X-ray free-electron laser

    Energy Technology Data Exchange (ETDEWEB)

    Kroll, Thomas; Kern, Jan; Kubin, Markus; Ratner, Daniel; Gul, Sheraz; Fuller, Franklin D.; Löchel, Heike; Krzywinski, Jacek; Lutman, Alberto; Ding, Yuantao; Dakovski, Georgi L.; Moeller, Stefan; Turner, Joshua J.; Alonso-Mori, Roberto; Nordlund, Dennis L.; Rehanek, Jens; Weniger, Christian; Firsov, Alexander; Brzhezinskaya, Maria; Chatterjee, Ruchira; Lassalle-Kaiser, Benedikt; Sierra, Raymond G.; Laksmono, Hartawan; Hill, Ethan; Borovik, Andrew; Erko, Alexei; Föhlisch, Alexander; Mitzner, Rolf; Yachandra, Vittal K.; Yano, Junko; Wernet, Philippe; Bergmann, Uwe

    2016-01-01

    © 2016 Optical Society of America. X-ray free electron lasers (XFELs) enable unprecedented new ways to study the electronic structure and dynamics of transition metal systems. L-edge absorption spectroscopy is a powerful technique for such studies and the feasibility of this method at XFELs for solutions and solids has been demonstrated. However, the required x-ray bandwidth is an order of magnitude narrower than that of self-amplified spontaneous emission (SASE), and additional monochromatization is needed. Here we compare L-edge x-ray absorption spectroscopy (XAS) of a prototypical transition metal system based on monochromatizing the SASE radiation of the linac coherent light source (LCLS) with a new technique based on self-seeding of LCLS. We demonstrate how L-edge XAS can be performed using the self-seeding scheme without the need of an additional beam line monochromator. We show how the spectral shape and pulse energy depend on the undulator setup and how this affects the x-ray spectroscopy measurements.

  12. Inner-shell photo-ionized X-ray laser schemes for low-Z elements

    International Nuclear Information System (INIS)

    Moon, S.J.; Strobel, G.L.

    1994-01-01

    Gain calculations for inner-shell photo-ionized lasing in C at 45 angstrom are performed. An incident x-ray source represented by a 150 eV blackbody with a rise time of 50 fsec gives a gain of order 10 cm -1 . The x-ray source and thus the driving optical laser requirements are significantly reduced as compared to what is needed for Ne at 15 angstrom. The authors expect that existing ultra-short pulse lasers can produce the required x-ray source and thus produce a table-top x-ray laser at 45 angstrom

  13. The trickle before the torrent-diffraction data from X-ray lasers.

    Science.gov (United States)

    Maia, Filipe R N C; Hajdu, Janos

    2016-08-01

    Today Scientific Data launched a collection of publications describing data from X-ray free-electron lasers under the theme 'Structural Biology Applications of X-ray Lasers'. The papers cover data on nanocrystals, single virus particles, isolated cell organelles, and living cells. All data are deposited with the Coherent X-ray Imaging Data Bank (CXIDB) and available to the scientific community to develop ideas, tools and procedures to meet challenges with the expected torrents of data from new X-ray lasers, capable of producing billion exposures per day.

  14. Time-resolved hard x-ray studies using third-generation synchrotron radiation sources (abstract)

    International Nuclear Information System (INIS)

    Mills, D.M.

    1992-01-01

    The third-generation, high-brilliance, synchrotron radiation sources currently under construction will usher in a new era of x-ray research in the physical, chemical, and biological sciences. One of the most exciting areas of experimentation will be the extension of static x-ray scattering and diffraction techniques to the study of transient or time-evolving systems. The high repetition rate, short-pulse duration, high-brilliance, variable spectral bandwidth, and large particle beam energies of these sources make them ideal for hard x-ray, time-resolved studies. The primary focus of this presentation will be on the novel instrumentation required for time-resolved studies such as optics which can increase the flux on the sample or disperse the x-ray beam, detectors and electronics for parallel data collection, and methods for altering the natural time structure of the radiation. This work is supported by the U.S. Department of Energy, BES-Materials Science, under Contract No. W-31-109-ENG-38

  15. Laser interaction with matter as a source of U.V. and soft X-ray radiation: application to X-ray cinematography

    International Nuclear Information System (INIS)

    Tonon, G.F.; Colombant, Denis; Delmare, Claude; Rabeau, Maxime

    A new detecting device is described. It allows one to get the frequency, the time and space resolution of pictures of U.V. and soft X ray emission of a laser created plasma in a single shot: X ray pictures of such a plasma are presented. After these preliminary results, it is possible to set up readily an X ray framing camera. A laser created plasma is an X ray source of special interest: the emitted power can be 10% of the laser intensity and the emitted spectrum is centered around 1A wavelength [fr

  16. Evaluating scintillator performance in time-resolved hard X-ray studies at synchrotron light sources

    International Nuclear Information System (INIS)

    Rutherford, Michael E.; Chapman, David J.; White, Thomas G.; Drakopoulos, Michael; Rack, Alexander; Eakins, Daniel E.

    2016-01-01

    Scintillator performance in time-resolved, hard, indirect detection X-ray studies on the sub-microsecond timescale at synchrotron light sources is reviewed, modelled and examined experimentally. LYSO:Ce is found to be the only commercially available crystal suitable for these experiments. The short pulse duration, small effective source size and high flux of synchrotron radiation is ideally suited for probing a wide range of transient deformation processes in materials under extreme conditions. In this paper, the challenges of high-resolution time-resolved indirect X-ray detection are reviewed in the context of dynamic synchrotron experiments. In particular, the discussion is targeted at two-dimensional integrating detector methods, such as those focused on dynamic radiography and diffraction experiments. The response of a scintillator to periodic synchrotron X-ray excitation is modelled and validated against experimental data collected at the Diamond Light Source (DLS) and European Synchrotron Radiation Facility (ESRF). An upper bound on the dynamic range accessible in a time-resolved experiment for a given bunch separation is calculated for a range of scintillators. New bunch structures are suggested for DLS and ESRF using the highest-performing commercially available crystal LYSO:Ce, allowing time-resolved experiments with an interframe time of 189 ns and a maximum dynamic range of 98 (6.6 bits)

  17. Evaluating scintillator performance in time-resolved hard X-ray studies at synchrotron light sources

    Energy Technology Data Exchange (ETDEWEB)

    Rutherford, Michael E.; Chapman, David J.; White, Thomas G. [Imperial College London, London (United Kingdom); Drakopoulos, Michael [Diamond Light Source, I12 Joint Engineering, Environmental, Processing (JEEP) Beamline, Didcot, Oxfordshire (United Kingdom); Rack, Alexander [European Synchrotron Radiation Facility, Grenoble (France); Eakins, Daniel E., E-mail: d.eakins@imperial.ac.uk [Imperial College London, London (United Kingdom)

    2016-03-24

    Scintillator performance in time-resolved, hard, indirect detection X-ray studies on the sub-microsecond timescale at synchrotron light sources is reviewed, modelled and examined experimentally. LYSO:Ce is found to be the only commercially available crystal suitable for these experiments. The short pulse duration, small effective source size and high flux of synchrotron radiation is ideally suited for probing a wide range of transient deformation processes in materials under extreme conditions. In this paper, the challenges of high-resolution time-resolved indirect X-ray detection are reviewed in the context of dynamic synchrotron experiments. In particular, the discussion is targeted at two-dimensional integrating detector methods, such as those focused on dynamic radiography and diffraction experiments. The response of a scintillator to periodic synchrotron X-ray excitation is modelled and validated against experimental data collected at the Diamond Light Source (DLS) and European Synchrotron Radiation Facility (ESRF). An upper bound on the dynamic range accessible in a time-resolved experiment for a given bunch separation is calculated for a range of scintillators. New bunch structures are suggested for DLS and ESRF using the highest-performing commercially available crystal LYSO:Ce, allowing time-resolved experiments with an interframe time of 189 ns and a maximum dynamic range of 98 (6.6 bits)

  18. Development of a compact x-ray source via laser compton scattering at KEK-LUCX

    International Nuclear Information System (INIS)

    Sakaue, Kazuyuki; Washio, Masakazu; Aryshev, Alexander; Araki, Sakae; Urakawa, Junji; Terunuma, Nobuhiro; Fukuda, Masafumi; Miyoshi, Toshinobu; Takeda, Ayaki

    2013-01-01

    The compact X-ray source based on Laser-Compton scattering (LCS) has been developed at LUCX (Laser Undulator Compact X-ray source) facility in KEK. The multi-bunch high quality electron beam produced by a standing wave 3.6 cell RF Gun and accelerated by the followed S-band normal conducting 12 cells standing wave 'Booster' linear accelerator is scattered off the laser beam stored in the optical cavity. The 4-mirror planar optical cavity with finesse 335 is used. The MCP (Micro-Channer Plate) detector as well as SOI (Silicon-On-Insulator) pixel sensor was used for scattered X-ray detection. The SOI pixel sensor has been used for LCS X-ray detection for the first time and has demonstrated high spatial resolution and high SN ratio X-ray detection that in turn lead to clearest X-ray images achieved by LCS X-ray. We have also achieved generation of 6.38x10 6 ph./sec., which is more than 30 times larger LCS X-ray flux in comparison with our previous results. The complete details of LUCX LCS X-ray source, specifications of both electron and laser beams, and the results of LCS X-ray generation experiments are reported in this paper. (author)

  19. Numerical Simulations of X-Ray Free Electron Lasers (XFEL)

    KAUST Repository

    Antonelli, Paolo

    2014-11-04

    We study a nonlinear Schrödinger equation which arises as an effective single particle model in X-ray free electron lasers (XFEL). This equation appears as a first principles model for the beam-matter interactions that would take place in an XFEL molecular imaging experiment in [A. Fratalocchi and G. Ruocco, Phys. Rev. Lett., 106 (2011), 105504]. Since XFEL are more powerful by several orders of magnitude than more conventional lasers, the systematic investigation of many of the standard assumptions and approximations has attracted increased attention. In this model the electrons move under a rapidly oscillating electromagnetic field, and the convergence of the problem to an effective time-averaged one is examined. We use an operator splitting pseudospectral method to investigate numerically the behavior of the model versus that of its time-averaged version in complex situations, namely the energy subcritical/mass supercritical case and in the presence of a periodic lattice. We find the time-averaged model to be an effective approximation, even close to blowup, for fast enough oscillations of the external field. This work extends previous analytical results for simpler cases [P. Antonelli, A. Athanassoulis, H. Hajaiej, and P. Markowich, Arch. Ration. Mech. Anal., 211 (2014), pp. 711--732].

  20. Optically-ionized plasma recombination x-ray lasers

    International Nuclear Information System (INIS)

    Amendt, P.; Eder, D.C.; Wilks, S.C.; Dunning, M.J.; Keane, C.J.

    1991-01-01

    Design studies for recombination x-ray lasers based on plasmas ionized by high intensity, short pulse optical lasers are presented. Transient lasing on n = 3 to n = 2 transitions in Lithium-like Neon allows for moderately short wavelengths (≤ 100 angstrom) without requiring ionizing intensities associated with relativistic electron quiver energies. The electron energy distribution following the ionizing pulse affects directly the predicted gains for this resonance transition. Efficiencies of 10 -6 or greater are found for plasma temperatures in the vicinity of 40 eV. Simulation studies of parametric heating phenomena relating to stimulated Raman and Compton scattering are presented. For electron densities less than about 2.5 x 10 20 cm -3 and peak driver intensity of 2 x 10 17 W/cm 2 at 0.25 μm with pulse length of 100 fsec, the amount of electron heating is found to be marginally significant. For Lithium-like Aluminum, the required relativistic ionizing intensity gives excessive electron heating and reduced efficiency, thereby rendering this scheme impractical for generating shorter wavelength lasing (≤ 50 angstrom) in the transient case. Following the transient lasing phase, a slow hydrodynamic expansion into the surrounding cool plasma is accompanied by quasi-static gain on the n = 4 to n = 3 transition in Lithium-like Neon. Parametric heating effects on gain optimization in this regime are also discussed. 18 refs., 6 figs

  1. Cytogenetic studies with laser or X-ray exposures

    International Nuclear Information System (INIS)

    Bozduganov, A.; Genkov, P.

    1975-01-01

    Account is given of studies involving a total of 21 peripheral blood cultures given the following treatments: exposure to 20 0.13-joule pulses from an optic quantum generator (ruby), 9; exposure to 1000 R X-rays, 9; and unexposed controls, 3. Exposures were carried out on three cultures from each experimental series at each of three time intervals, namely 24 h, 48 h, and 72 h after initiation of cultures. On any day, 40 well-spread metaphases were examined. High quality metaphases were photographed and karyotyped in conformity to the Chicago Conference criteria. In the laser experiment, chromosome aberrations were observed in 65% of methaphases analyzed vs. 5.3% in controls. Anomalies encountered included aneuploidy, with hypoploid metaphases predominating, polyploidy (triploidy, tetraploidy, and partial endoreduplication), and structural alterations. The following structural chromosome rearrangements are found: acentric fragments, mostly pairs, occasionally single, including minute chromosomes; dicentric and tricentric chromosomes; interstitial deletions; and chromosome translocations. Most varied and abundant chromosome aberrations were seen in 72-h irradiated cultures. The data presented offer a new opportunity for assessing genetic lesions after laser exposure and may help to determine threshold doses. (author)

  2. Novel technique for spatially resolved imaging of molecular bond orientations using x-ray birefringence

    Energy Technology Data Exchange (ETDEWEB)

    Sutter, John P., E-mail: john.sutter@diamond.ac.uk; Dolbnya, Igor P.; Collins, Stephen P. [Diamond Light Source Ltd, Harwell Science and Innovation Campus, Chilton, Didcot, Oxfordshire OX11 0DE (United Kingdom); Harris, Kenneth D. M., E-mail: HarrisKDM@cardiff.ac.uk; Edwards-Gau, Gregory R.; Kariuki, Benson M. [School of Chemistry, Cardiff University, Park Place, Cardiff CF10 3AT (United Kingdom); Palmer, Benjamin A. [Department of Structural Biology, Weizmann Institute of Science, 234 Herzl St., Rehovot 7610001 (Israel)

    2016-07-27

    Birefringence has been observed in anisotropic materials transmitting linearly polarized X-ray beams tuned close to an absorption edge of a specific element in the material. Synchrotron bending magnets provide X-ray beams of sufficiently high brightness and cross section for spatially resolved measurements of birefringence. The recently developed X-ray Birefringence Imaging (XBI) technique has been successfully applied for the first time using the versatile test beamline B16 at Diamond Light Source. Orientational distributions of the C–Br bonds of brominated “guest” molecules within crystalline “host” tunnel structures (in thiourea or urea inclusion compounds) have been studied using linearly polarized incident X-rays near the Br K-edge. Imaging of domain structures, changes in C–Br bond orientations associated with order-disorder phase transitions, and the effects of dynamic averaging of C–Br bond orientations have been demonstrated. The XBI setup uses a vertically deflecting high-resolution double-crystal monochromator upstream from the sample and a horizontally deflecting single-crystal polarization analyzer downstream, with a Bragg angle as close as possible to 45°. In this way, the ellipticity and rotation angle of the polarization of the beam transmitted through the sample is measured as in polarizing optical microscopy. The theoretical instrumental background calculated from the elliptical polarization of the bending-magnet X-rays, the imperfect polarization discrimination of the analyzer, and the correlation between vertical position and photon energy introduced by the monochromator agrees well with experimental observations. The background is calculated analytically because the region of X-ray phase space selected by this setup is sampled inefficiently by standard methods.

  3. Time resolved resonant inelastic X-ray scattering: A supreme tool to understand dynamics in solids and molecules

    International Nuclear Information System (INIS)

    Beye, M.; Wernet, Ph.; Schüßler-Langeheine, C.; Föhlisch, A.

    2013-01-01

    Highlights: •The high specificity of RIXS ideally suits time-resolved measurements. •Methods relating to the core hole lifetime cover the low femtosecond regime. •Pump-probe methods are used starting at sub-ps time scales. •FELs and synchrotrons are useful for pump-probe studies. •Examples from solid state dynamics and molecules are discussed. -- Abstract: Dynamics in materials typically involve different degrees of freedom, like charge, lattice, orbital and spin in a complex interplay. Time-resolved resonant inelastic X-ray scattering (RIXS) as a highly selective tool can provide unique insight and follow the details of dynamical processes while resolving symmetries, chemical and charge states, momenta, spin configurations, etc. In this paper, we review examples where the intrinsic scattering duration time is used to study femtosecond phenomena. Free-electron lasers access timescales starting in the sub-ps range through pump-probe methods and synchrotrons study the time scales longer than tens of ps. In these examples, time-resolved resonant inelastic X-ray scattering is applied to solids as well as molecular systems

  4. X-ray streak-camera study of the dynamics of laser-imploded microballoons

    International Nuclear Information System (INIS)

    Key, M.H.; Lamb, M.J.; Lewis, C.L.S.; Moore, A.; Evans, R.G.

    1979-01-01

    The time and space development of the x-ray emission from the irradiated target surface and the implosion core in laser-compressed glass microballoons is recorded by x-ray streak photography. The experimental variation of implosion time with target mass and laser energy is considered and compared with computer modeling of the implosion

  5. A system for time-resolved x-ray diffraction and its application to muscle contraction

    International Nuclear Information System (INIS)

    Amemiya, Yoshiyuki; Hashizume, Hiroo.

    1979-01-01

    A data-collection system has been built which permits time-resolved studies of X-ray diffraction diagrams obtained from contracting muscle on millisecond time scale. The system consists of a linear delay-line position sensitive proportional counter (PSPC), a special data transfer unit and an on-line computer. The PSPC used with a mirror-monochromator camera can detect equatorial reflections from stimulated muscle in a total exposure time of a few seconds. Time-resolved data-collection is achieved by stimulating muscle at a regular time interval, dividing a complete cycle of muscle contraction into many successive time slices and accumulating in computer memory X-ray data for each time slice from many repeated cycles of stimulation. The performances of the system have been demonstrated by recording equatorial reflections from frog skeletal muscle during isometric and isotonic twitch with a time resolution of 25 ms. (author)

  6. Time-resolved measurements of supersonic fuel sprays using synchrotron x-rays

    International Nuclear Information System (INIS)

    Powell, C.F.; Yue, Y.; Poola, R.; Wang, J.

    2000-11-01

    A time-resolved radiographic technique has been developed for probing the fuel distribution close to the nozzle of a high-pressure single-hole diesel injector. The measurement was made using X-ray absorption of monochromatic synchrotron-generated radiation, allowing quantitative determination of the fuel distribution in this optically impenetrable region with a time resolution of better than 1 μs. These quantitative measurements constitute the most detailed near-nozzle study of a fuel spray to date

  7. Time-resolved measurements of supersonic fuel sprays using synchrotron X-rays.

    Science.gov (United States)

    Powell, C F; Yue, Y; Poola, R; Wang, J

    2000-11-01

    A time-resolved radiographic technique has been developed for probing the fuel distribution close to the nozzle of a high-pressure single-hole diesel injector. The measurement was made using X-ray absorption of monochromatic synchrotron-generated radiation, allowing quantitative determination of the fuel distribution in this optically impenetrable region with a time resolution of better than 1 micros. These quantitative measurements constitute the most detailed near-nozzle study of a fuel spray to date.

  8. Development and characterization of a laser-based hard x-ray source

    International Nuclear Information System (INIS)

    Tillman, C.

    1996-11-01

    A laser-produced plasma was generated by focusing 100 fs laser pulses, with an energy of 150 mJ, onto metal targets. The laser intensity was expected to reach 10 17 W/cm -2 . Radiation was emitted from the created plasma, with photon energies up to the MeV region. The laser-based X-ray source was optimized, with the purpose of making it a realistic source of hard X-rays (>10 keV). Dedicated equipment was developed for efficient generation and utilization of the hard X-rays. The X-ray source was characterized with respect to its spatial extent and the X-ray yield. Measurements were made of the spectral distribution, by the use of single-photon-counting detectors in different geometries, crystal spectrometers and dose measurements in combination with absorption filters. Ablation of the target material in the laser produced plasma was investigated. Imaging applications have been demonstrated, including ultrafast (picosecond) X-ray imaging, magnification imaging of up to x80, differential imaging in the spectral domain, and imaging of various biological and technical objects. The biological response of ultra-intense X-ray pulses was assessed in cell-culture exposures. The results indicate that the biological response from ultra-intense X-ray exposures is similar to the response with conventional X-ray tubes. 82 refs., 14 figs

  9. Development and characterization of a laser-based hard x-ray source

    Energy Technology Data Exchange (ETDEWEB)

    Tillman, C.

    1996-11-01

    A laser-produced plasma was generated by focusing 100 fs laser pulses, with an energy of 150 mJ, onto metal targets. The laser intensity was expected to reach 10{sup 17} W/cm{sup -2}. Radiation was emitted from the created plasma, with photon energies up to the MeV region. The laser-based X-ray source was optimized, with the purpose of making it a realistic source of hard X-rays (>10 keV). Dedicated equipment was developed for efficient generation and utilization of the hard X-rays. The X-ray source was characterized with respect to its spatial extent and the X-ray yield. Measurements were made of the spectral distribution, by the use of single-photon-counting detectors in different geometries, crystal spectrometers and dose measurements in combination with absorption filters. Ablation of the target material in the laser produced plasma was investigated. Imaging applications have been demonstrated, including ultrafast (picosecond) X-ray imaging, magnification imaging of up to x80, differential imaging in the spectral domain, and imaging of various biological and technical objects. The biological response of ultra-intense X-ray pulses was assessed in cell-culture exposures. The results indicate that the biological response from ultra-intense X-ray exposures is similar to the response with conventional X-ray tubes. 82 refs., 14 figs.

  10. High power, short pulses ultraviolet laser for the development of a new x-ray laser

    International Nuclear Information System (INIS)

    Meixler, L.; Nam, C.H.; Robinson, J.; Tighe, W.; Krushelnick, K.; Suckewer, S.; Goldhar, J.; Seely, J.; Feldman, U.

    1989-04-01

    A high power, short pulse ultraviolet laser system (Powerful Picosecond-Laser) has been developed at the Princeton Plasma Physics Laboratory (PPPL) as part of experiments designed to generate shorter wavelength x-ray lasers. With the addition of pulse compression and a final KrF amplifier the laser output is expected to have reached 1/3-1/2 TW (10 12 watts) levels. The laser system, particularly the final amplifier, is described along with some initial soft x-ray spectra from laser-target experiments. The front end of the PP-Laser provides an output of 20--30 GW (10 9 watts) and can be focussed to intensities of /approximately/10 16 W/cm 2 . Experiments using this output to examine the effects of a prepulse on laser-target interaction are described. 19 refs., 14 figs

  11. X-ray emission as a potential hazard during ultrashort pulse laser material processing

    Science.gov (United States)

    Legall, Herbert; Schwanke, Christoph; Pentzien, Simone; Dittmar, Günter; Bonse, Jörn; Krüger, Jörg

    2018-06-01

    In laser machining with ultrashort laser pulses unwanted X-ray radiation in the keV range can be generated when a critical laser intensity is exceeded. Even if the emitted X-ray dose per pulse is low, high laser repetition rates can lead to an accumulation of X-ray doses beyond exposure safety limits. For 925 fs pulse duration at a center wavelength of 1030 nm, the X-ray emission was investigated up to an intensity of 2.6 × 1014 W/cm2. The experiments were performed in air with a thin disk laser at a repetition rate of 400 kHz. X-ray spectra and doses were measured for various planar target materials covering a wide range of the periodic table from aluminum to tungsten. Without radiation shielding, the measured radiation doses at this high repetition rate clearly exceed the regulatory limits. Estimations for an adequate radiation shielding are provided.

  12. UV-Visible Absorption Spectroscopy Enhanced X-ray Crystallography at Synchrotron and X-ray Free Electron Laser Sources.

    Science.gov (United States)

    Cohen, Aina E; Doukov, Tzanko; Soltis, Michael S

    2016-01-01

    This review describes the use of single crystal UV-Visible Absorption micro-Spectrophotometry (UV-Vis AS) to enhance the design and execution of X-ray crystallography experiments for structural investigations of reaction intermediates of redox active and photosensitive proteins. Considerations for UV-Vis AS measurements at the synchrotron and associated instrumentation are described. UV-Vis AS is useful to verify the intermediate state of an enzyme and to monitor the progression of reactions within crystals. Radiation induced redox changes within protein crystals may be monitored to devise effective diffraction data collection strategies. An overview of the specific effects of radiation damage on macromolecular crystals is presented along with data collection strategies that minimize these effects by combining data from multiple crystals used at the synchrotron and with the X-ray free electron laser.

  13. Soft x-ray emission from postpulse expanding laser-produced plasmas

    International Nuclear Information System (INIS)

    Weaver, J.L.; Feldman, U.; Mostovych, A.N.; Seely, J.F.; Colombant, D.; Holland, G.

    2003-01-01

    A diagnostic spectrometer has been developed at the Naval Research Laboratory to measure the time resolved absolute intensity of radiation emitted from targets irradiated by the Nike laser. The spectrometer consists of a dispersive transmission grating of 2500 lines/mm or 5000 lines/mm and a detection system consisting of an absolutely calibrated Si photodiode array and a charge coupled device camera. In this article, this spectrometer was used to study the spatial distribution of soft x-ray radiation from low Z elements (primarily carbon) that lasted tens of nanoseconds after the main laser illumination was over. We recorded soft x-ray emission as a function of the target material and target orientation with respect to the incoming laser beam and the spectrometer line of sight. While a number of spectral features have been identified in the data, the instrument's combined temporal and spatial resolution allowed observation of the plasma expansion from CH targets for up to ∼25 ns after the cessation of the main laser pulse. The inferred plasma expansion velocities are slightly higher than those previously reported

  14. Soft x-ray emission from postpulse expanding laser-produced plasmas

    Science.gov (United States)

    Weaver, J. L.; Feldman, U.; Mostovych, A. N.; Seely, J. F.; Colombant, D.; Holland, G.

    2003-12-01

    A diagnostic spectrometer has been developed at the Naval Research Laboratory to measure the time resolved absolute intensity of radiation emitted from targets irradiated by the Nike laser. The spectrometer consists of a dispersive transmission grating of 2500 lines/mm or 5000 lines/mm and a detection system consisting of an absolutely calibrated Si photodiode array and a charge coupled device camera. In this article, this spectrometer was used to study the spatial distribution of soft x-ray radiation from low Z elements (primarily carbon) that lasted tens of nanoseconds after the main laser illumination was over. We recorded soft x-ray emission as a function of the target material and target orientation with respect to the incoming laser beam and the spectrometer line of sight. While a number of spectral features have been identified in the data, the instrument's combined temporal and spatial resolution allowed observation of the plasma expansion from CH targets for up to ˜25 ns after the cessation of the main laser pulse. The inferred plasma expansion velocities are slightly higher than those previously reported.

  15. X-ray spectrometer having 12 000 resolving power at 8 keV energy

    Science.gov (United States)

    Seely, John F.; Hudson, Lawrence T.; Henins, Albert; Feldman, Uri

    2017-10-01

    An x-ray spectrometer employing a thin (50 μm) silicon transmission crystal was used to record high-resolution Cu Kα spectra from a laboratory x-ray source. The diffraction was from the (331) planes that were at an angle of 13.26° to the crystal surface. The components of the spectral lines resulting from single-vacancy (1s) and double-vacancy (1s and 3d) transitions were observed. After accounting for the natural lifetime widths from reference double-crystal spectra and the spatial resolution of the image plate detector, the intrinsic broadening of the transmission crystal was measured to be as small as 0.67 eV and the resolving power 12 000, the highest resolving power achieved by a compact (0.5 m long) spectrometer employing a single transmission crystal operating in the hard x-ray region. By recording spectra with variable source-to-crystal distances and comparing to the calculated widths from various geometrical broadening mechanisms, the primary contributions to the intrinsic crystal broadening were found to be the source height at small distances and the crystal apertured height at large distances. By reducing these two effects, using a smaller source size and vignetting the crystal height, the intrinsic crystal broadening is then limited by the crystal thickness and the rocking curve width and would be 0.4 eV at 8 keV energy (20 000 resolving power).

  16. Measuring the x-ray resolving power of bent potassium acid phthalate diffraction crystals

    International Nuclear Information System (INIS)

    Haugh, M. J.; Jacoby, K. D.; Wu, M.; Loisel, G. P.

    2014-01-01

    This report presents the results from measuring the X-ray resolving power of a curved potassium acid phthalate (KAP(001)) spectrometer crystal using two independent methods. It is part of a continuing effort to measure the fundamental diffraction properties of bent crystals that are used to study various characteristics of high temperature plasmas. Bent crystals like KAP(001) do not usually have the same diffraction properties as corresponding flat crystals. Models that do exist to calculate the effect of bending the crystal on the diffraction properties have simplifying assumptions and their accuracy limits have not been adequately determined. The type of crystals that we measured is being used in a spectrometer on the Z machine at Sandia National Laboratories in Albuquerque, New Mexico. The first technique for measuring the crystal resolving power measures the X-ray spectral line width of the characteristic lines from several metal anodes. The second method uses a diode X-ray source and a double crystal diffractometer arrangement to measure the reflectivity curve of the KAP(001) crystal. The width of that curve is inversely proportional to the crystal resolving power. The measurement results are analyzed and discussed

  17. Measuring the x-ray resolving power of bent potassium acid phthalate diffraction crystals

    Energy Technology Data Exchange (ETDEWEB)

    Haugh, M. J., E-mail: haughmj@nv.doe.gov; Jacoby, K. D. [National Security Technologies, LLC, Livermore, California 94550 (United States); Wu, M.; Loisel, G. P. [Sandia National Laboratories, Albuquerque, New Mexico 87123 (United States)

    2014-11-15

    This report presents the results from measuring the X-ray resolving power of a curved potassium acid phthalate (KAP(001)) spectrometer crystal using two independent methods. It is part of a continuing effort to measure the fundamental diffraction properties of bent crystals that are used to study various characteristics of high temperature plasmas. Bent crystals like KAP(001) do not usually have the same diffraction properties as corresponding flat crystals. Models that do exist to calculate the effect of bending the crystal on the diffraction properties have simplifying assumptions and their accuracy limits have not been adequately determined. The type of crystals that we measured is being used in a spectrometer on the Z machine at Sandia National Laboratories in Albuquerque, New Mexico. The first technique for measuring the crystal resolving power measures the X-ray spectral line width of the characteristic lines from several metal anodes. The second method uses a diode X-ray source and a double crystal diffractometer arrangement to measure the reflectivity curve of the KAP(001) crystal. The width of that curve is inversely proportional to the crystal resolving power. The measurement results are analyzed and discussed.

  18. Laser plasmas as x-ray sources for lithographic imaging of submicron structures

    International Nuclear Information System (INIS)

    Bijkerk, F.; van Dorssen, G.E.; van der Wiel, M.J.

    1988-01-01

    Laser radiation can be used efficiently to generate x-rays for lithographic imaging of submicron patterns, e.g., for VLSI device fabrication. Due to their short wavelength and high average power, excimer lasers show much potential for this application. Results are presented of scaling studies for high repetition rate excimer laser application, using the frequency doubled output of a low repetition rate Nd:YAG/Glass laser. Spectral and spatial characteristics of x-ray emission of the laser plasma are shown. The power density in the laser focus was 3 x 10 12 W/cm 2 . With this source Si x-ray masks with submicron Au absorber profiles are imaged into high sensitivity x-ray photoresist. For the exposures 80 laser shots sufficed to yield high quality submicron structures. Extrapolation of the results to a high power excimer laser reduces the exposure time of the photoresists to several seconds, enabling a wafer throughput at an industrial level

  19. Target focusing configuration for X-ray laser experiments

    International Nuclear Information System (INIS)

    Seppala, L.G.

    1985-01-01

    X-ray laser experiments imposed a new demand on the Novette focusing optics. These optics had to provide highly uniform, double-sided illumination on a target region 1.0 cm long by 100 to 200 μm wide. This line focus requirement had to be achieved without degrading the diagnostic reflection from the last surface of the focus lens and without potential ghost focus problems. The only optical configuration that preserves the diagnostic reflection is shown. A negative focal length cylinder lens is placed between the focus lens and the debris shield, with the concave surface facing toward the focus lens. Any ghost reflections from the cylinder lens or debris shield are degraded by astigmatism, making them less hazardous. In practice, the uniformity of illumination is probably about the same for a positive or a negative cylinder lens. The minimum Novette focused spot was approximately 50 to 75 μm in diameter, and the fabrication errors in the 80-cm-diam precision cylinder lens produced a line focus 25 μm wide. a negative cylinder lens design was chosen, however, to optimize the illumination uniformity in the case of line widths of several hundred microns

  20. Towards shorter wavelength x-ray lasers using a high power, short pulse pump laser

    International Nuclear Information System (INIS)

    Tighe, W.; Krushelnick, K.; Valeo, E.; Suckewer, S.

    1991-05-01

    A near-terawatt, KrF* laser system, focussable to power densities >10 18 W/cm 2 has been constructed for use as a pump laser in various schemes aimed at the development of x-ray lasing below 5nm. The laser system along with output characteristics such as the pulse duration, the focal spot size, and the percentage of amplified spontaneous emission (ASE) emitted along with the laser pulse will be presented. Schemes intended to lead to shorter wavelength x-ray emission will be described. The resultant requirements on the pump laser characteristics and the target design will be outlined. Results from recent solid target experiments and two-laser experiments, showing the interaction of a high-power, short pulse laser with a preformed plasma, will be presented. 13 refs., 5 figs

  1. Time-resolved X-ray transmission microscopy on magnetic microstructures; Zeitaufloesende Roentgentransmissionsmikroskopie an magnetischen Mikrostrukturen

    Energy Technology Data Exchange (ETDEWEB)

    Puzic, Aleksandar

    2007-10-23

    Three excitation schemes were designed for stroboscopic imaging of magnetization dynamics with time-resolved magnetic transmission X-ray microscopy (TR-MTXM). These techniques were implemented into two types of X-ray microscopes, namely the imaging transmission X-ray microscope (ITXM) and the scanning transmission X-ray microscope (STXM), both installed at the electron storage ring of the Advanced Light Source in Berkeley, USA. Circular diffraction gratings (Fresnel zone plates) used in both microscopes as focusing and imaging elements presently allow for lateral resolution down to 30 nm. Magnetic imaging is performed by using the X-ray magnetic circular dichroism (XMCD) as element specific contrast mechanism. The developed methods have been successfully applied to the experimental investigation of magnetization dynamics in ferromagnetic microstructures. A temporal resolution well below 100 ps was achieved. A conventional pump-probe technique was implemented first. The dynamic response of the magnetization excited by a broadband pulsed magnetic field was imaged spatially resolved using focused X-ray flashes. As a complementary method, the spatially resolved ferromagnetic resonance (SR-FMR) technique was developed for experimental study of magnetization dynamics in the frequency domain. As a third excitation mode, the burst excitation was implemented. The performance and efficiency of the developed methods have been demonstrated by imaging the local magnetization dynamics in laterally patterned ferromagnetic thin-film elements and three-layer stacks. The existence of multiple eigenmodes in the excitation spectra of ferromagnetic microstructures has been verified by using the pump-probe technique. Magnetostatic spin waves were selectively excited and detected with a time resolution of 50 ps using the SR-FMR technique. Thorough analysis of 20 in most cases independently prepared samples has verified that vortices which exhibit a low-amplitude switching of their core

  2. Time-resolved X-ray transmission microscopy on magnetic microstructures

    International Nuclear Information System (INIS)

    Puzic, Aleksandar

    2007-01-01

    Three excitation schemes were designed for stroboscopic imaging of magnetization dynamics with time-resolved magnetic transmission X-ray microscopy (TR-MTXM). These techniques were implemented into two types of X-ray microscopes, namely the imaging transmission X-ray microscope (ITXM) and the scanning transmission X-ray microscope (STXM), both installed at the electron storage ring of the Advanced Light Source in Berkeley, USA. Circular diffraction gratings (Fresnel zone plates) used in both microscopes as focusing and imaging elements presently allow for lateral resolution down to 30 nm. Magnetic imaging is performed by using the X-ray magnetic circular dichroism (XMCD) as element specific contrast mechanism. The developed methods have been successfully applied to the experimental investigation of magnetization dynamics in ferromagnetic microstructures. A temporal resolution well below 100 ps was achieved. A conventional pump-probe technique was implemented first. The dynamic response of the magnetization excited by a broadband pulsed magnetic field was imaged spatially resolved using focused X-ray flashes. As a complementary method, the spatially resolved ferromagnetic resonance (SR-FMR) technique was developed for experimental study of magnetization dynamics in the frequency domain. As a third excitation mode, the burst excitation was implemented. The performance and efficiency of the developed methods have been demonstrated by imaging the local magnetization dynamics in laterally patterned ferromagnetic thin-film elements and three-layer stacks. The existence of multiple eigenmodes in the excitation spectra of ferromagnetic microstructures has been verified by using the pump-probe technique. Magnetostatic spin waves were selectively excited and detected with a time resolution of 50 ps using the SR-FMR technique. Thorough analysis of 20 in most cases independently prepared samples has verified that vortices which exhibit a low-amplitude switching of their core

  3. A development of laser-plasma-based soft x-ray microscope system

    International Nuclear Information System (INIS)

    Nam, Ki Yong; Kim, Kyong Woo; Kim, Kyu Gyeom; Kwon, Young Man; Yoon, Kwon Ha

    2003-01-01

    Soft x-ray nano-imaging microscopy system for biomedical application with a high resolution about 50 nm has been designed and described, and its integrated techniques also have been studied. The system is mainly composed of soft x-ray generation system, nano-scaled control system, x-ray optical device like a condenser or object mirror, a CCD camera coupled with multichannel plate (MCP) and vacuum system. In the system, soft x-ray is generated from the laser-based plasma by focusing Nd:YAG laser beam on tantalum (Ta) target. In an x-ray optical system, a wolter mirror has been considering condensing the x-ray beam on a biological specimen and zone plate was adapted as an object mirror. A Si 3 N 4 was used as specimen holder for keeping a biological sample alive in atmosphere conditions. A back-illuminated-CCD camera coupled with multichannel plate was determined to set up.

  4. Metrology for X-ray lasers; Metrologie fuer Roentgenlaser

    Energy Technology Data Exchange (ETDEWEB)

    Richter, Mathias [Physikalisch-Technische Bundesanstalt (PTB), Berlin (Germany). Fachbereich ' Radiometrie mit Synchrotronstrahlung' ; Gottwald, Alexander; Krumrey, Michael

    2014-09-15

    With free-electron lasers pulse-resolved experiments can be performed. In this article gas-monitor detectors are described, which are based on photoionization and can be used for real-time studies in such experiments. An experimental setup with a time-of-flight spectrometer is described, and the results on Xe-ion spectra obtained with this setup at a photon energy of 93 eV are presented. (HSI)

  5. ANALYSIS AND MITIGATION OF X-RAY HAZARD GENERATED FROM HIGH INTENSITY LASER-TARGET INTERACTIONS

    Energy Technology Data Exchange (ETDEWEB)

    Qiu, R.; Liu, J.C.; Prinz, A.A.; Rokni, S.H.; Woods, M.; Xia, Z.; /SLAC

    2011-03-21

    Interaction of a high intensity laser with matter may generate an ionizing radiation hazard. Very limited studies have been made, however, on the laser-induced radiation protection issue. This work reviews available literature on the physics and characteristics of laser-induced X-ray hazards. Important aspects include the laser-to-electron energy conversion efficiency, electron angular distribution, electron energy spectrum and effective temperature, and bremsstrahlung production of X-rays in the target. The possible X-ray dose rates for several femtosecond Ti:sapphire laser systems used at SLAC, including the short pulse laser system for the Matter in Extreme Conditions Instrument (peak power 4 TW and peak intensity 2.4 x 10{sup 18} W/cm{sup 2}) were analysed. A graded approach to mitigate the laser-induced X-ray hazard with a combination of engineered and administrative controls is also proposed.

  6. Characteristics of X-ray photons in tilted incident laser-produced plasma

    International Nuclear Information System (INIS)

    Wang Ruirong; Chen Weimin; Xie Dongzhu

    2008-01-01

    Characteristics of X-ray and spout direction of heat plasma flow were studied on Shenguang-II laser facility. Using of pinhole X-ray camera, X-ray photons from the plasma of aluminum (Al) irradiated by 1.053 μm laser, was measured and analysed. It is observed that the spatial distribution of X-ray photons in Al plasma for tilted irradiation is symmetic at the center of the target. The spout direction of heat plasma flow is inferred by the distribution contour of X-ray photons. the experimental results show that the spout direction of heat plasma flow is normal to target plane and the output intensity of X-ray photons does not increase significantly for tilted laser incidence. Uniformity of laser energy deposition is improved by superposing tilted incident and laser perpendicularly incident laser. At the same time, it is found that the conversion efficiency from the tilted incident laser energy to X-ray photons of laser-produced plasma is decreased. (authors)

  7. Absolute Soft X-ray Emission Measurements at the Nike Laser

    Science.gov (United States)

    Weaver, J.; Atkin, R.; Boyer, C.; Colombant, D.; Feldman, U.; Fielding, D.; Gardner, J.; Holland, G.; Klapisch, M.; Mostovych, A. N.; Obenscain, S.; Seely, J. F.

    2002-11-01

    Recent experiments at the Nike laser facility have demonstrated that, when a low intensity prepulse ( 2main laser intensity) is used to heat a thin Au or Pd coating on a planar CH target, the growth of non-uniformities due to laser imprint can be reduced from the growth observed for an uncoated CH target. The absolute radiation intensity in the soft x-ray region (0.1-1 keV) has a important role in the energy balance for layered targets. There is an ongoing effort to characterize the soft x-ray emission using an absolutely calibrated transmission grating spectrometer and filtered diode modules. Measurements of the angular distribution of the emission from unlayered solid targets (Au, Pd, CH) have recently been made using an array of moveable filtered diode modules. The data from the angular distribution studies will be presented. A new absolutely calibrated, time-resolving transmission grating spectrometer has been installed at the Nike. The new version has improved spectral resolution, selectable transmission filters, and the potential for simultaneous temporal, spatial, and spectral resolution. Preliminary data from the new spectrometer will be presented and future experiments will be briefly discussed. *Work was supported by DoE

  8. Direct measurements of multi-photon induced nonlinear lattice dynamics in semiconductors via time-resolved x-ray scattering.

    Science.gov (United States)

    Williams, G Jackson; Lee, Sooheyong; Walko, Donald A; Watson, Michael A; Jo, Wonhuyk; Lee, Dong Ryeol; Landahl, Eric C

    2016-12-22

    Nonlinear optical phenomena in semiconductors present several fundamental problems in modern optics that are of great importance for the development of optoelectronic devices. In particular, the details of photo-induced lattice dynamics at early time-scales prior to carrier recombination remain poorly understood. We demonstrate the first integrated measurements of both optical and structural, material-dependent quantities while also inferring the bulk impulsive strain profile by using high spatial-resolution time-resolved x-ray scattering (TRXS) on bulk crystalline gallium arsenide. Our findings reveal distinctive laser-fluence dependent crystal lattice responses, which are not described by previous TRXS experiments or models. The initial linear expansion of the crystal upon laser excitation stagnates at a laser fluence corresponding to the saturation of the free carrier density before resuming expansion in a third regime at higher fluences where two-photon absorption becomes dominant. Our interpretations of the lattice dynamics as nonlinear optical effects are confirmed by numerical simulations and by additional measurements in an n-type semiconductor that allows higher-order nonlinear optical processes to be directly observed as modulations of x-ray diffraction lineshapes.

  9. Study of compact X-ray laser pumped by pulse-train laser. Double-target experiment

    International Nuclear Information System (INIS)

    Yamaguchi, Naohiro; Fujikawa, Chiemi; Hara, Tamio

    2000-01-01

    We have been developing a tabletop x-ray laser based on the recombination plasma scheme. An advanced experiment has been started to improve x-ray laser output substantially. Two 11-mm-long laser produced plasmas were produced so that their axis aligned into a line, the double-target configuration. X-ray intensity of the 15.47 nm transition line of the Li-like Al ion has been enhanced in the double-target configuration. (author)

  10. Diagnostics of underwater electrical wire explosion through a time- and space-resolved hard x-ray source.

    Science.gov (United States)

    Sheftman, D; Shafer, D; Efimov, S; Gruzinsky, K; Gleizer, S; Krasik, Ya E

    2012-10-01

    A time- and space-resolved hard x-ray source was developed as a diagnostic tool for imaging underwater exploding wires. A ~4 ns width pulse of hard x-rays with energies of up to 100 keV was obtained from the discharge in a vacuum diode consisting of point-shaped tungsten electrodes. To improve contrast and image quality, an external pulsed magnetic field produced by Helmholtz coils was used. High resolution x-ray images of an underwater exploding wire were obtained using a sensitive x-ray CCD detector, and were compared to optical fast framing images. Future developments and application of this diagnostic technique are discussed.

  11. Attosecond time-energy structure of X-ray free-electron laser pulses

    Science.gov (United States)

    Hartmann, N.; Hartmann, G.; Heider, R.; Wagner, M. S.; Ilchen, M.; Buck, J.; Lindahl, A. O.; Benko, C.; Grünert, J.; Krzywinski, J.; Liu, J.; Lutman, A. A.; Marinelli, A.; Maxwell, T.; Miahnahri, A. A.; Moeller, S. P.; Planas, M.; Robinson, J.; Kazansky, A. K.; Kabachnik, N. M.; Viefhaus, J.; Feurer, T.; Kienberger, R.; Coffee, R. N.; Helml, W.

    2018-04-01

    The time-energy information of ultrashort X-ray free-electron laser pulses generated by the Linac Coherent Light Source is measured with attosecond resolution via angular streaking of neon 1s photoelectrons. The X-ray pulses promote electrons from the neon core level into an ionization continuum, where they are dressed with the electric field of a circularly polarized infrared laser. This induces characteristic modulations of the resulting photoelectron energy and angular distribution. From these modulations we recover the single-shot attosecond intensity structure and chirp of arbitrary X-ray pulses based on self-amplified spontaneous emission, which have eluded direct measurement so far. We characterize individual attosecond pulses, including their instantaneous frequency, and identify double pulses with well-defined delays and spectral properties, thus paving the way for X-ray pump/X-ray probe attosecond free-electron laser science.

  12. Supersonic Heat Wave Propagation in Laser-Produced Underdense Plasma for Efficient X-Ray Generation

    International Nuclear Information System (INIS)

    Tanabe, M.; Nishimura, H.; Fujioka, S.; Nagai, K.; Iwamae, A.; Ohnishi, N.; Fournier, K.B.; Girard, F.; Primout, M.; Villette, B.; Tobin, M.; Mima, K.

    2008-01-01

    We have observed supersonic heat wave propagation in a low-density aerogel target (ρ ∼ 3.2 mg/cc) irradiated at the intensity of 4 x 10 14 W/cm 2 . The heat wave propagation was measured with a time-resolved x-ray imaging diagnostics, and the results were compared with simulations made with the two-dimensional radiation-hydrodynamic code, RAICHO. Propagation velocity of the ionization front gradually decreased as the wave propagates into the target. The reason of decrease is due to increase of laser absorption region as the front propagates and interplay of hydrodynamic motion and reflection of laser propagation. These features are well reported with the simulation

  13. AN OSCILLATOR CONFIGURATION FOR FULL REALIZATION OF HARD X-RAY FREE ELECTRON LASER*

    Energy Technology Data Exchange (ETDEWEB)

    Kim, K.-J.; Kolodziej, T.; Lindberg, R. R.; Shu, D.; Shvyd' ko, Y.; Stoupin, S.; Maxwell, T.J.; Ding, Y.; Fawley, W. M.; Hastings, J.; Huang, Z; Krzywinski, J.; Marcus, G.; Qin, Weilun; Medvedev, N.; Zemella, J.; Blank, V.; Terentyev, S.

    2017-06-01

    An x-ray free electron laser oscillator (XFELO) is feasible by employing an X-ray cavity with Bragg mirrors such as diamond crystals. An XFELO at the 5th harmonic frequency may be implemented at the LCLS II using its 4 GeV superconducting linac, producing stable, fully coherent, high-spectral-purity hard x-rays. In addition, its output can be a coherent seed to the LCLS amplifier for stable, high-power, femto-second x-ray pulses. We summarize the recent progress in various R&D efforts addressing critical issues for realizing an XFELO at LCLS II.

  14. Soft-X-Ray Projection Lithography Using a High-Repetition-Rate Laser-Induced X-Ray Source for Sub-100 Nanometer Lithography Processes

    NARCIS (Netherlands)

    E. Louis,; F. Bijkerk,; Shmaenok, L.; Voorma, H. J.; van der Wiel, M. J.; Schlatmann, R.; Verhoeven, J.; van der Drift, E. W. J. M.; Romijn, J.; Rousseeuw, B. A. C.; Voss, F.; Desor, R.; Nikolaus, B.

    1993-01-01

    In this paper we present the status of a joint development programme on soft x-ray projection lithography (SXPL) integrating work on high brightness laser plasma sources. fabrication of multilayer x-ray mirrors. and patterning of reflection masks. We are in the process of optimization of a

  15. Study Of Soot Growth And Nucleation By A Time-Resolved Synchrotron Radiation Based X-Ray Absorption Method

    National Research Council Canada - National Science Library

    Mitchell, Judith I

    2001-01-01

    This report results from a contract tasking University of Rennes I as follows: The contractor will perform a study of soot growth and nucleation by a time-resolved synchrotron radiation based x-ray absorption method...

  16. X-ray diodes for laser fusion plasma diagnostics

    International Nuclear Information System (INIS)

    Day, R.H.; Lee, P.; Saloman, E.B.; Nagel, D.J.

    1981-02-01

    Photodiodes with x-ray sensitive photocathodes are commonly used as broadband x-ray detectors in fusion plasma diagnostics. We have measured the risetime of the detector system and have measured the quantum efficiency between 1 to 500 A of numerous photocathode materials of practical interest. The materials studied include aluminum, copper, nickel, gold, three forms of carbon, chromium, and cesium iodide. The results of the measurements are compared with Henke's semiempirical model of photoyield. We have studied the effects of long-term cathode aging and use as a plasma diagnostic on cathode quantum efficiency. In addition, we have measured the x-ray mass-absorption coefficient of several ultrasoft x-ray windows in energy regions where data were unavailable. Windows studied were made of aluminum, Formvar, polypropylene, and Kimfoil. Measurements between 1 to 50 A were performed with the Los Alamos Scientific Laboratory's low-energy x-ray calibration facility, and the measurements between 50 to 550 A were performed at the National Bureau of Standard's synchrotron ultraviolet radiation facility

  17. Time-resolved x-ray diffraction techniques for bulk polycrystalline materials under dynamic loading

    Energy Technology Data Exchange (ETDEWEB)

    Lambert, P. K.; Hustedt, C. J.; Zhao, M.; Ananiadis, A. G.; Hufnagel, T. C. [Department of Materials Science and Engineering, Johns Hopkins University, Baltimore, Maryland 21218 (United States); Vecchio, K. S. [Department of NanoEngineering, University of California San Diego, La Jolla, California 92093 (United States); Huskins, E. L. [Oak Ridge Institute for Science and Education, Oak Ridge, Tennessee 37830 (United States); US Army Research Laboratory, Aberdeen Proving Ground, Aberdeen, Maryland 21005 (United States); Casem, D. T. [US Army Research Laboratory, Aberdeen Proving Ground, Aberdeen, Maryland 21005 (United States); Gruner, S. M. [Department of Physics, Cornell University, Ithaca, New York 14853 (United States); Cornell High Energy Synchrotron Source (CHESS), Cornell University, Ithaca, New York 14853 (United States); Kavli Institute at Cornell for Nanoscale Science, Cornell University, Ithaca, New York 14853 (United States); Tate, M. W.; Philipp, H. T.; Purohit, P.; Weiss, J. T. [Department of Physics, Cornell University, Ithaca, New York 14853 (United States); Woll, A. R. [Cornell High Energy Synchrotron Source (CHESS), Cornell University, Ithaca, New York 14853 (United States); Kannan, V.; Ramesh, K. T. [Department of Mechanical Engineering, Johns Hopkins University, Baltimore, Maryland 21218 (United States); Kenesei, P.; Okasinski, J. S.; Almer, J. [X-ray Science Division, Argonne National Laboratory, Argonne, Illinois 60439 (United States)

    2014-09-15

    We have developed two techniques for time-resolved x-ray diffraction from bulk polycrystalline materials during dynamic loading. In the first technique, we synchronize a fast detector with loading of samples at strain rates of ∼10{sup 3}–10{sup 4} s{sup −1} in a compression Kolsky bar (split Hopkinson pressure bar) apparatus to obtain in situ diffraction patterns with exposures as short as 70 ns. This approach employs moderate x-ray energies (10–20 keV) and is well suited to weakly absorbing materials such as magnesium alloys. The second technique is useful for more strongly absorbing materials, and uses high-energy x-rays (86 keV) and a fast shutter synchronized with the Kolsky bar to produce short (∼40 μs) pulses timed with the arrival of the strain pulse at the specimen, recording the diffraction pattern on a large-format amorphous silicon detector. For both techniques we present sample data demonstrating the ability of these techniques to characterize elastic strains and polycrystalline texture as a function of time during high-rate deformation.

  18. Novel energy resolving x-ray pinhole camera on Alcator C-Moda)

    Science.gov (United States)

    Pablant, N. A.; Delgado-Aparicio, L.; Bitter, M.; Brandstetter, S.; Eikenberry, E.; Ellis, R.; Hill, K. W.; Hofer, P.; Schneebeli, M.

    2012-10-01

    A new energy resolving x-ray pinhole camera has been recently installed on Alcator C-Mod. This diagnostic is capable of 1D or 2D imaging with a spatial resolution of ≈1 cm, an energy resolution of ≈1 keV in the range of 3.5-15 keV and a maximum time resolution of 5 ms. A novel use of a Pilatus 2 hybrid-pixel x-ray detector [P. Kraft et al., J. Synchrotron Rad. 16, 368 (2009), 10.1107/S0909049509009911] is employed in which the lower energy threshold of individual pixels is adjusted, allowing regions of a single detector to be sensitive to different x-ray energy ranges. Development of this new detector calibration technique was done as a collaboration between PPPL and Dectris Ltd. The calibration procedure is described, and the energy resolution of the detector is characterized. Initial data from this installation on Alcator C-Mod is presented. This diagnostic provides line-integrated measurements of impurity emission which can be used to determine impurity concentrations as well as the electron energy distribution.

  19. Single-particle coherent diffractive imaging with a soft x-ray free electron laser: towards soot aerosol morphology

    Science.gov (United States)

    Bogan, Michael J.; Starodub, Dmitri; Hampton, Christina Y.; Sierra, Raymond G.

    2010-10-01

    The first of its kind, the Free electron LASer facility in Hamburg, FLASH, produces soft x-ray pulses with unprecedented properties (10 fs, 6.8-47 nm, 1012 photons per pulse, 20 µm diameter). One of the seminal FLASH experiments is single-pulse coherent x-ray diffractive imaging (CXDI). CXDI utilizes the ultrafast and ultrabright pulses to overcome resolution limitations in x-ray microscopy imposed by x-ray-induced damage to the sample by 'diffracting before destroying' the sample on sub-picosecond timescales. For many lensless imaging algorithms used for CXDI it is convenient when the data satisfy an oversampling constraint that requires the sample to be an isolated object, i.e. an individual 'free-standing' portion of disordered matter delivered to the centre of the x-ray focus. By definition, this type of matter is an aerosol. This paper will describe the role of aerosol science methodologies used for the validation of the 'diffract before destroy' hypothesis and the execution of the first single-particle CXDI experiments being developed for biological imaging. FLASH CXDI now enables the highest resolution imaging of single micron-sized or smaller airborne particulate matter to date while preserving the native substrate-free state of the aerosol. Electron microscopy offers higher resolution for single-particle analysis but the aerosol must be captured on a substrate, potentially modifying the particle morphology. Thus, FLASH is poised to contribute significant advancements in our knowledge of aerosol morphology and dynamics. As an example, we simulate CXDI of combustion particle (soot) morphology and introduce the concept of extracting radius of gyration of fractal aggregates from single-pulse x-ray diffraction data. Future upgrades to FLASH will enable higher spatially and temporally resolved single-particle aerosol dynamics studies, filling a critical technological need in aerosol science and nanotechnology. Many of the methodologies described for FLASH will

  20. Space and time resolved spectroscopy of laser-produced plasmas: A study of density-sensitive x-ray transitions in helium-like and neon-like ions

    International Nuclear Information System (INIS)

    Young, Bruce Kai Fong.

    1988-09-01

    The determination of level populations and detailed population mechanisms in dense plasmas has become an increasingly important problem in atomic physics. In this work, the density variation of line intensities and level populations in aluminum K-shell and molybdenum and silver L-shell emission spectra have been measured from high-powered, laser-produced plasmas. For each case, the density dependence of the observed line emission is due to the effect of high frequency electron-ion collisions on metastable levels. The density dependent line intensities vary greatly in laser-produced plasmas and can be used to extract detailed information concerning the population kinetics and level populations of the ions. The laser-plasmas had to be fully characterized in order to clearly compare the observed density dependence with atomic theory predictions. This has been achieved through the combined use of new diagnostic instruments and microdot targets which provided simultaneously space, time, and spectrally resolved data. The plasma temperatures were determined from the slope of the hydrogen-like recombination continuum. The time resolved electron density profiles were measured using multiple frame holographic interferometry. Thus, the density dependence of K-shell spectral lines could be clearly examined, independent of assumptions concerning the dynamics of the plasma. In aluminum, the electron density dependence of various helium-like line intensity ratios were measured. Standard collisional radiative equilibrium models fail to account for the observed density dependence measured for the ''He/sub α//IC'' ratio. Instead, a quasi-steady state atomic model based on a purely recombining plasma is shown to accurately predict the measured density dependence. This same recombining plasma calculation successfully models the density dependence of the high-n ''He/sub γ//He/sub β/'' and ''He/sub δ//He/sub β/'' helium-like resonance line intensity ratios

  1. Space and time resolved spectroscopy of laser-produced plasmas: A study of density-sensitive x-ray transitions in helium-like and neon-like ions

    Energy Technology Data Exchange (ETDEWEB)

    Young, Bruce Kai Fong

    1988-09-01

    The determination of level populations and detailed population mechanisms in dense plasmas has become an increasingly important problem in atomic physics. In this work, the density variation of line intensities and level populations in aluminum K-shell and molybdenum and silver L-shell emission spectra have been measured from high-powered, laser-produced plasmas. For each case, the density dependence of the observed line emission is due to the effect of high frequency electron-ion collisions on metastable levels. The density dependent line intensities vary greatly in laser-produced plasmas and can be used to extract detailed information concerning the population kinetics and level populations of the ions. The laser-plasmas had to be fully characterized in order to clearly compare the observed density dependence with atomic theory predictions. This has been achieved through the combined use of new diagnostic instruments and microdot targets which provided simultaneously space, time, and spectrally resolved data. The plasma temperatures were determined from the slope of the hydrogen-like recombination continuum. The time resolved electron density profiles were measured using multiple frame holographic interferometry. Thus, the density dependence of K-shell spectral lines could be clearly examined, independent of assumptions concerning the dynamics of the plasma. In aluminum, the electron density dependence of various helium-like line intensity ratios were measured. Standard collisional radiative equilibrium models fail to account for the observed density dependence measured for the ''He/sub ..cap alpha..//IC'' ratio. Instead, a quasi-steady state atomic model based on a purely recombining plasma is shown to accurately predict the measured density dependence. This same recombining plasma calculation successfully models the density dependence of the high-n ''He/sub ..gamma..//He/sub ..beta../'' and ''He/sub delta

  2. Evaluating scintillator performance in time-resolved hard X-ray studies at synchrotron light sources.

    Science.gov (United States)

    Rutherford, Michael E; Chapman, David J; White, Thomas G; Drakopoulos, Michael; Rack, Alexander; Eakins, Daniel E

    2016-05-01

    The short pulse duration, small effective source size and high flux of synchrotron radiation is ideally suited for probing a wide range of transient deformation processes in materials under extreme conditions. In this paper, the challenges of high-resolution time-resolved indirect X-ray detection are reviewed in the context of dynamic synchrotron experiments. In particular, the discussion is targeted at two-dimensional integrating detector methods, such as those focused on dynamic radiography and diffraction experiments. The response of a scintillator to periodic synchrotron X-ray excitation is modelled and validated against experimental data collected at the Diamond Light Source (DLS) and European Synchrotron Radiation Facility (ESRF). An upper bound on the dynamic range accessible in a time-resolved experiment for a given bunch separation is calculated for a range of scintillators. New bunch structures are suggested for DLS and ESRF using the highest-performing commercially available crystal LYSO:Ce, allowing time-resolved experiments with an interframe time of 189 ns and a maximum dynamic range of 98 (6.6 bits).

  3. Particle tracking during Ostwald ripening using time-resolved laboratory X-ray microtomography

    Energy Technology Data Exchange (ETDEWEB)

    Werz, T., E-mail: thomas.werz@uni-ulm.de [Ulm University, Institute of Micro and Nanomaterials, Albert-Einstein-Allee 47, 89081 (Germany); Baumann, M. [Ulm University, Institute of Micro and Nanomaterials, Albert-Einstein-Allee 47, 89081 (Germany); Wolfram, U. [Ulm University, Institute of Orthopaedic Research and Biomechanics, Helmholtzstrasse 14, 89081 (Germany); Krill, C.E. [Ulm University, Institute of Micro and Nanomaterials, Albert-Einstein-Allee 47, 89081 (Germany)

    2014-04-01

    Laboratory X-ray microtomography is investigated as a method for obtaining time-resolved images of microstructural coarsening of the semisolid state of Al–5 wt.% Cu samples during Ostwald ripening. Owing to the 3D imaging capability of tomography, this technique uniquely provides access to the growth rates of individual particles, thereby not only allowing a statistical characterization of coarsening—as has long been possible by conventional metallography—but also enabling quantification of the influence of local environment on particle boundary migration. The latter information is crucial to understanding growth kinetics during Ostwald ripening at high volume fractions of the coarsening phase. Automated image processing and segmentation routines were developed to close gaps in the network of particle boundaries and to track individual particles from one annealing step to the next. The particle tracking success rate places an upper bound of only a few percent on the likelihood of segmentation errors for any given particle. The accuracy of particle size trajectories extracted from the time-resolved tomographic reconstructions is correspondingly high. Statistically averaged coarsening data and individual particle growth rates are in excellent agreement with the results of prior experimental studies and with computer simulations of Ostwald ripening. - Highlights: • Ostwald ripening in Al–5 wt.% Cu measured by laboratory X-ray microtomography • Time-resolved measurement of individual particle growth • Automated segmentation routines developed to close gaps in particle boundary network • Particle growth/shrinkage rates deviate from LSW model prediction.

  4. Atomic motion of resonantly vibrating quartz crystal visualized by time-resolved X-ray diffraction

    International Nuclear Information System (INIS)

    Aoyagi, Shinobu; Osawa, Hitoshi; Sugimoto, Kunihisa; Fujiwara, Akihiko; Takeda, Shoichi; Moriyoshi, Chikako; Kuroiwa, Yoshihiro

    2015-01-01

    Transient atomic displacements during a resonant thickness-shear vibration of AT-cut α-quartz are revealed by time-resolved X-ray diffraction under an alternating electric field. The lattice strain resonantly amplified by the alternating electric field is ∼10 4 times larger than that induced by a static electric field. The resonantly amplified lattice strain is achieved by fast displacements of oxygen anions and collateral resilient deformation of Si−O−Si angles bridging rigid SiO 4 tetrahedra, which efficiently transduce electric energy into elastic energy

  5. Shielded radiography with a laser-driven MeV-energy X-ray source

    Energy Technology Data Exchange (ETDEWEB)

    Chen, Shouyuan; Golovin, Grigory [Department of Physics and Astronomy, University of Nebraska-Lincoln, Lincoln, NE 68588 (United States); Miller, Cameron [Department of Nuclear Engineering and Radiological Sciences, University of Michigan, Ann Arbor, MI 48109 (United States); Haden, Daniel; Banerjee, Sudeep; Zhang, Ping; Liu, Cheng; Zhang, Jun; Zhao, Baozhen [Department of Physics and Astronomy, University of Nebraska-Lincoln, Lincoln, NE 68588 (United States); Clarke, Shaun; Pozzi, Sara [Department of Nuclear Engineering and Radiological Sciences, University of Michigan, Ann Arbor, MI 48109 (United States); Umstadter, Donald, E-mail: donald.umstadter@unl.edu [Department of Physics and Astronomy, University of Nebraska-Lincoln, Lincoln, NE 68588 (United States)

    2016-01-01

    We report the results of experimental and numerical-simulation studies of shielded radiography using narrowband MeV-energy X-rays from a compact all-laser-driven inverse-Compton-scattering X-ray light source. This recently developed X-ray light source is based on a laser-wakefield accelerator with ultra-high-field gradient (GeV/cm). We demonstrate experimentally high-quality radiographic imaging (image contrast of 0.4 and signal-to-noise ratio of 2:1) of a target composed of 8-mm thick depleted uranium shielded by 80-mm thick steel, using a 6-MeV X-ray beam with a spread of 45% (FWHM) and 10{sup 7} photons in a single shot. The corresponding dose of the X-ray pulse measured in front of the target is ∼100 nGy/pulse. Simulations performed using the Monte-Carlo code MCNPX accurately reproduce the experimental results. These simulations also demonstrate that the narrow bandwidth of the Compton X-ray source operating at 6 and 9 MeV leads to a reduction of deposited dose as compared to broadband bremsstrahlung sources with the same end-point energy. The X-ray beam’s inherently low-divergence angle (∼mrad) is advantageous and effective for interrogation at standoff distance. These results demonstrate significant benefits of all-laser driven Compton X-rays for shielded radiography.

  6. Instantaneous x-ray radiation energy from laser produced polystyrene plasmas for shock ignition conditions

    International Nuclear Information System (INIS)

    Shang, Wanli; Wei, Huiyue; Li, Zhichao; Yi, Rongqing; Zhu, Tuo; Song, Tianmin; Huang, Chengwu; Yang, Jiamin

    2013-01-01

    Laser target energy coupling mechanism is crucial in the shock ignition (SI) scheme, and x-ray radiation energy is a non-negligible portion of the laser produced plasma energy. To evaluate the x-ray radiation energy amount at conditions relevant to SI scheme, instantaneous x-ray radiation energy is investigated experimentally with continuum phase plates smoothed lasers irradiating layer polystyrene targets. Comparative laser pulses without and with shock spike are employed. With the measured x-ray angular distribution, full space x-ray radiation energy and conversion efficiency are observed. Instantaneous scaling law of x-ray conversion efficiency is obtained as a function of laser intensity and time. It should be pointed out that the scaling law is available for any laser pulse shape and intensity, with which irradiates polystyrene planar target with intensity from 2 × 10 14 to 1.8 × 10 15 W/cm 2 . Numerical analysis of the laser energy transformation is performed, and the simulation results agree with the experimental data

  7. Computational time-resolved and resonant x-ray scattering of strongly correlated materials

    Energy Technology Data Exchange (ETDEWEB)

    Bansil, Arun [Northeastern Univ., Boston, MA (United States)

    2016-11-09

    predominantly decays via Auger processes, thereby providing an internal time-scale, which limits intermediate-state processes to timescales of a few femtoseconds. Accordingly, a number of activities directed at modeling K-, L- and M-edge RIXS in correlated materials were also pursused by our CRT. Our research effort supported by this CMCSN grant substantially advanced the understanding of x-ray scattering processes in the time-domain as well as in the more conventional scattering channels, including time-resolved photoemission, and how such processes can be modeled realistically in complex correlated materials more generally. The modeling of relaxation processes involved in time-domain spectroscopies is important also for understanding photoinduced effects such as energy conversion in photosynthesis and solar cell applications, and thus impacts the basic science for energy needs.

  8. Ultraviolet laser transverse profile shaping for improving x-ray free electron laser performance

    International Nuclear Information System (INIS)

    Li, S.; Alverson, S.; Bohler, D.; Egger, A.; Fry, A.

    2017-01-01

    The photocathode rf gun is one of the most critical components in x-ray free electron lasers. The drive laser strikes the photocathode surface, which emits electrons with properties that depend on the shape of the drive laser. Most free electron lasers use photocathodes with work function in the ultraviolet, a wavelength where direct laser manipulation becomes challenging. In this paper, we present a novel application of a digital micromirror device (DMD) for the 253 nm drive laser at the Linear Coherent Light Source. Laser profile shaping is accomplished through an iterative algorithm that takes into account shaping error and efficiency. Next, we use laser shaping to control the X-ray laser output via an online optimizer, which shows improvement in FEL pulse energy. Lastly, as a preparation for electron beam shaping, we use the DMD to measure the photocathode quantum efficiency across cathode surface with an averaged laser rms spot size of 59 μm. In conclusion, our experiments demonstrate promising outlook of using DMD to shape ultraviolet lasers for photocathode rf guns with various applications.

  9. Ultraviolet laser transverse profile shaping for improving x-ray free electron laser performance

    Science.gov (United States)

    Li, S.; Alverson, S.; Bohler, D.; Egger, A.; Fry, A.; Gilevich, S.; Huang, Z.; Miahnahri, A.; Ratner, D.; Robinson, J.; Zhou, F.

    2017-08-01

    The photocathode rf gun is one of the most critical components in x-ray free electron lasers. The drive laser strikes the photocathode surface, which emits electrons with properties that depend on the shape of the drive laser. Most free electron lasers use photocathodes with work function in the ultraviolet, a wavelength where direct laser manipulation becomes challenging. In this paper, we present a novel application of a digital micromirror device (DMD) for the 253 nm drive laser at the Linear Coherent Light Source. Laser profile shaping is accomplished through an iterative algorithm that takes into account shaping error and efficiency. Next, we use laser shaping to control the X-ray laser output via an online optimizer, which shows improvement in FEL pulse energy. Lastly, as a preparation for electron beam shaping, we use the DMD to measure the photocathode quantum efficiency across cathode surface with an averaged laser rms spot size of 59 μ m . Our experiments demonstrate promising outlook of using DMD to shape ultraviolet lasers for photocathode rf guns with various applications.

  10. Characterization of diffraction gratings by use of a tabletop soft-x-ray laser

    International Nuclear Information System (INIS)

    Seminario, Max; Rocca, Jorge J.; Depine, Ricardo A.; Bach, Benny; Bach, Bernie

    2001-01-01

    We have demonstrated the use of a high-repetition-rate 46.9-mm tabletop laser to characterize diffraction gratings designed for grazing-incidence operation in the soft-x-ray spectral region. The efficiencies for various diffraction orders were measured as a function of angle of incidence and compared with the results of model simulations. This measurement technique provides benchmarks with which to improve electromagnetic codes used in the design of soft-x-ray diffraction gratings. The results illustrate the potential of compact tabletop soft-x-ray lasers for use as a new tool for characterization of short-wavelength optics at the manufacturer's site

  11. Progress in compact soft x-ray lasers and their applications

    International Nuclear Information System (INIS)

    Suckewer, S.; Skinner, C.H.

    1995-01-01

    The ultra-high brightness and short pulse duration of soft x-ray lasers provide unique advantages for novel applications. A crucial factor in the availability of these devices is their scale and cost. Recent breakthroughs in this field has brought closer the advent of table-top devices, suitable for applications to fields such as x-ray microscopy, chemistry, material science, plasma diagnostics, and lithography. In this article we review recent progress in the development of compact (table-top) soft x-ray lasers

  12. Laser power meters as an X-ray power diagnostic for LCLS-II.

    Science.gov (United States)

    Heimann, Philip; Moeller, Stefan; Carbajo, Sergio; Song, Sanghoon; Dakovski, Georgi; Nordlund, Dennis; Fritz, David

    2018-01-01

    For the LCLS-II X-ray instruments, laser power meters are being developed as compact X-ray power diagnostics to operate at soft and tender X-ray photon energies. These diagnostics can be installed at various locations along an X-ray free-electron laser (FEL) beamline in order to monitor the transmission of X-ray optics along the beam path. In addition, the power meters will be used to determine the absolute X-ray power at the endstations. Here, thermopile power meters, which measure average power, and have been chosen primarily for their compatibility with the high repetition rates at LCLS-II, are evaluated. A number of characteristics in the soft X-ray range are presented including linearity, calibrations conducted with a photodiode and a gas monitor detector as well as ultra-high-vacuum compatibility tests using residual gas analysis. The application of these power meters for LCLS-II and other X-ray FEL sources is discussed.

  13. X-ray calorimeters used for measurement in laser-fusion experiments

    International Nuclear Information System (INIS)

    Tang Daorun; China Academy of Engineering Physics, Mianyang; Wu Dengxue; Lin Libin; Sun Kexu; Jiang Shaoen

    2005-01-01

    X-ray calorimeters are ready to measure the total soft X-ray energy emitted from the plasma produced by laser because of their bodily absorption, linear response, insensitivity to the electromagnetic disturbance, and so on. The calorimeters mainly include absorbers, thermocouples, bases and shrouds. When X-rays are deposited in the absorbers, photon energy absorbed is quickly converted into intrinsic energy which simultaneously dissipates by thermal conduction and radiation. The X-ray calorimeters were absolutely on-line calibrated in Shenguang-II laser facility with the X-ray diode array spectrometer which has been absolutely calibrated on Beijing Synchrotron Radiation Facility. 20 shots' experimental results show that the X-ray calorimeters are stable, the sensitivity of calorimeter is (84.1 ± 3.4) μv/mJ and the related combined standard uncertainty in the X-ray energy measure is about 31%. The calorimeters can be applied to measure the X-ray energy. (authors)

  14. Time-resolved x-ray absorption spectroscopy: Watching atoms dance

    Science.gov (United States)

    Milne, Chris J.; Pham, Van-Thai; Gawelda, Wojciech; van der Veen, Renske M.; El Nahhas, Amal; Johnson, Steven L.; Beaud, Paul; Ingold, Gerhard; Lima, Frederico; Vithanage, Dimali A.; Benfatto, Maurizio; Grolimund, Daniel; Borca, Camelia; Kaiser, Maik; Hauser, Andreas; Abela, Rafael; Bressler, Christian; Chergui, Majed

    2009-11-01

    The introduction of pump-probe techniques to the field of x-ray absorption spectroscopy (XAS) has allowed the monitoring of both structural and electronic dynamics of disordered systems in the condensed phase with unprecedented accuracy, both in time and in space. We present results on the electronically excited high-spin state structure of an Fe(II) molecular species, [FeII(bpy)3]2+, in aqueous solution, resolving the Fe-N bond distance elongation as 0.2 Å. In addition an analysis technique using the reduced χ2 goodness of fit between FEFF EXAFS simulations and the experimental transient absorption signal in energy space has been successfully tested as a function of excited state population and chemical shift, demonstrating its applicability in situations where the fractional excited state population cannot be determined through other measurements. Finally by using a novel ultrafast hard x-ray 'slicing' source the question of how the molecule relaxes after optical excitation has been successfully resolved using femtosecond XANES.

  15. Ultra high-speed x-ray imaging of laser-driven shock compression using synchrotron light

    Science.gov (United States)

    Olbinado, Margie P.; Cantelli, Valentina; Mathon, Olivier; Pascarelli, Sakura; Grenzer, Joerg; Pelka, Alexander; Roedel, Melanie; Prencipe, Irene; Laso Garcia, Alejandro; Helbig, Uwe; Kraus, Dominik; Schramm, Ulrich; Cowan, Tom; Scheel, Mario; Pradel, Pierre; De Resseguier, Thibaut; Rack, Alexander

    2018-02-01

    A high-power, nanosecond pulsed laser impacting the surface of a material can generate an ablation plasma that drives a shock wave into it; while in situ x-ray imaging can provide a time-resolved probe of the shock-induced material behaviour on macroscopic length scales. Here, we report on an investigation into laser-driven shock compression of a polyurethane foam and a graphite rod by means of single-pulse synchrotron x-ray phase-contrast imaging with MHz frame rate. A 6 J, 10 ns pulsed laser was used to generate shock compression. Physical processes governing the laser-induced dynamic response such as elastic compression, compaction, pore collapse, fracture, and fragmentation have been imaged; and the advantage of exploiting the partial spatial coherence of a synchrotron source for studying low-density, carbon-based materials is emphasized. The successful combination of a high-energy laser and ultra high-speed x-ray imaging using synchrotron light demonstrates the potentiality of accessing complementary information from scientific studies of laser-driven shock compression.

  16. Developments in time-resolved high pressure x-ray diffraction using rapid compression and decompression

    International Nuclear Information System (INIS)

    Smith, Jesse S.; Sinogeikin, Stanislav V.; Lin, Chuanlong; Rod, Eric; Bai, Ligang; Shen, Guoyin

    2015-01-01

    Complementary advances in high pressure research apparatus and techniques make it possible to carry out time-resolved high pressure research using what would customarily be considered static high pressure apparatus. This work specifically explores time-resolved high pressure x-ray diffraction with rapid compression and/or decompression of a sample in a diamond anvil cell. Key aspects of the synchrotron beamline and ancillary equipment are presented, including source considerations, rapid (de)compression apparatus, high frequency imaging detectors, and software suitable for processing large volumes of data. A number of examples are presented, including fast equation of state measurements, compression rate dependent synthesis of metastable states in silicon and germanium, and ultrahigh compression rates using a piezoelectric driven diamond anvil cell

  17. Coherent Sources of XUV Radiation Soft X-Ray Lasers and High-Order Harmonic Generation

    CERN Document Server

    Jaeglé, Pierre

    2006-01-01

    Extreme ultraviolet radiation, also referred to as soft X-rays or XUV, offers very special optical properties. The X-UV refractive index of matter is such that normal reflection cannot take place on polished surfaces whereas beam transmission through one micrometer of almost all materials reduces to zero. Therefore, it has long been a difficult task to imagine and to implement devices designed for complex optics experiments in this wavelength range. Thanks to new sources of coherent radiation - XUV-lasers and High Order Harmonics - the use of XUV radiation, for interferometry, holography, diffractive optics, non-linear radiation-matter interaction, time-resolved study of fast and ultrafast phenomena and many other applications, including medical sciences, is ubiquitous.

  18. Picosecond x-ray streak camera studies

    International Nuclear Information System (INIS)

    Kasyanov, Yu.S.; Malyutin, A.A.; Richardson, M.C.; Chevokin, V.K.

    1975-01-01

    Some initial results of direct measurement of picosecond x-ray emission from laser-produced plasmas are presented. A PIM-UMI 93 image converter tube, incorporating an x-ray sensitive photocathode, linear deflection, and three stages of image amplification was used to analyse the x-ray radiation emanating from plasmas produced from solid Ti targets by single high-intensity picosecond laser pulses. From such plasmas, the x-ray emission typically persisted for times of 60psec. However, it is shown that this detection system should be capable of resolving x-ray phenomena of much shorter duration. (author)

  19. X ray emission: a tool and a probe for laser - clusters interaction

    International Nuclear Information System (INIS)

    Prigent, Ch.

    2004-12-01

    In intense laser-cluster interaction, the experimental results show a strong energetic coupling between radiation and matter. We have measured absolute X-ray yields and charge state distributions under well control conditions as a function of physical parameters governing the interaction; namely laser intensity, pulse duration, wavelength or polarization state of the laser light, the size and the species of the clusters (Ar, Kr, Xe). We have highlighted, for the first time, an intensity threshold in the X-ray production very low (∼ 2.10 14 W/cm 2 for a pulse duration of 300 fs) which can results from an effect of the dynamical polarisation of clusters in an intense electric field. A weak dependence with the wavelength (400 nm / 800 nm) on the absolute X-ray yields has been found. Moreover, we have observed a saturation of the X-ray emission probability below a critical cluster size. (author)

  20. Injection Methods and Instrumentation for Serial X-ray Free Electron Laser Experiments

    Science.gov (United States)

    James, Daniel

    Scientists have used X-rays to study biological molecules for nearly a century. Now with the X-ray free electron laser (XFEL), new methods have been developed to advance structural biology. These new methods include serial femtosecond crystallography, single particle imaging, solution scattering, and time resolved techniques. The XFEL is characterized by high intensity pulses, which are only about 50 femtoseconds in duration. The intensity allows for scattering from microscopic particles, while the short pulses offer a way to outrun radiation damage. XFELs are powerful enough to obliterate most samples in a single pulse. While this allows for a "diffract and destroy" methodology, it also requires instrumentation that can position microscopic particles into the X-ray beam (which may also be microscopic), continuously renew the sample after each pulse, and maintain sample viability during data collection. Typically these experiments have used liquid microjets to continuously renew sample. The high flow rate associated with liquid microjets requires large amounts of sample, most of which runs to waste between pulses. An injector designed to stream a viscous gel-like material called lipidic cubic phase (LCP) was developed to address this problem. LCP, commonly used as a growth medium for membrane protein crystals, lends itself to low flow rate jetting and so reduces the amount of sample wasted significantly. This work discusses sample delivery and injection for XFEL experiments. It reviews the liquid microjet method extensively, and presents the LCP injector as a novel device for serial crystallography, including detailed protocols for the LCP injector and anti-settler operation.

  1. Development of X-ray photoelectron microscope with a compact X-ray source generated by line-focused laser irradiation

    International Nuclear Information System (INIS)

    Yamaguchi, N.; Takahashi, Z.; Nishimura, Y.; Watanabe, K.; Okamoto, Y.; Sakata, A.; Azuma, H.; Hara, T.

    2005-01-01

    A laboratory-sized X-ray photoelectron microscope was constructed using a compact X-ray source produced by line-focused laser irradiation. The system is a scanning type photoelectron microscope where X-ray beam is micro-focused via Schwarzschild optics. A compact laser-plasma X-ray source has been developed with a YAG laser, a line-focus lens assembly, an Al tape-target driver and a debris prevention system. The 13.1 nm X-ray was delivered along line plasma whose length was 0.6 or 11 mm with higher intensity than that from a point-focused source. The Schwarzschild optics having the designed demagnification of 224, which was coated with Mo/Si multilayers for 13.1 nm X-ray, was set on the beamline 1 m distant from the source. The electron energy analyser was a spherical capacitor analyser with the photoelectron image detection system that was suited for detection of vast photoelectrons excited by an X-ray pulse of ns-order duration. The spatial resolution less than 5 μm has been confirmed from the variation of As 3d electron intensity along the position of the GaAs sample coated with a photo-resist test pattern

  2. Images of the laser entrance hole from the static x-ray imager at NIF.

    Science.gov (United States)

    Schneider, M B; Jones, O S; Meezan, N B; Milovich, J L; Town, R P; Alvarez, S S; Beeler, R G; Bradley, D K; Celeste, J R; Dixit, S N; Edwards, M J; Haugh, M J; Kalantar, D H; Kline, J L; Kyrala, G A; Landen, O L; MacGowan, B J; Michel, P; Moody, J D; Oberhelman, S K; Piston, K W; Pivovaroff, M J; Suter, L J; Teruya, A T; Thomas, C A; Vernon, S P; Warrick, A L; Widmann, K; Wood, R D; Young, B K

    2010-10-01

    The static x-ray imager at the National Ignition Facility is a pinhole camera using a CCD detector to obtain images of Hohlraum wall x-ray drive illumination patterns seen through the laser entrance hole (LEH). Carefully chosen filters, combined with the CCD response, allow recording images in the x-ray range of 3-5 keV with 60 μm spatial resolution. The routines used to obtain the apparent size of the backlit LEH and the location and intensity of beam spots are discussed and compared to predictions. A new soft x-ray channel centered at 870 eV (near the x-ray peak of a 300 eV temperature ignition Hohlraum) is discussed.

  3. Quantum theory for 1D X-ray free electron laser

    Science.gov (United States)

    Anisimov, Petr M.

    2018-06-01

    Classical 1D X-ray Free Electron Laser (X-ray FEL) theory has stood the test of time by guiding FEL design and development prior to any full-scale analysis. Future X-ray FELs and inverse-Compton sources, where photon recoil approaches an electron energy spread value, push the classical theory to its limits of applicability. After substantial efforts by the community to find what those limits are, there is no universally agreed upon quantum approach to design and development of future X-ray sources. We offer a new approach to formulate the quantum theory for 1D X-ray FELs that has an obvious connection to the classical theory, which allows for immediate transfer of knowledge between the two regimes. We exploit this connection in order to draw quantum mechanical conclusions about the quantum nature of electrons and generated radiation in terms of FEL variables.

  4. Mesoscopic structural phase progression in photo-excited VO2 revealed by time-resolved x-ray diffraction microscopy

    Science.gov (United States)

    Zhu, Yi; Cai, Zhonghou; Chen, Pice; Zhang, Qingteng; Highland, Matthew J.; Jung, Il Woong; Walko, Donald A.; Dufresne, Eric M.; Jeong, Jaewoo; Samant, Mahesh G.; Parkin, Stuart S. P.; Freeland, John W.; Evans, Paul G.; Wen, Haidan

    2016-02-01

    Dynamical phase separation during a solid-solid phase transition poses a challenge for understanding the fundamental processes in correlated materials. Critical information underlying a phase transition, such as localized phase competition, is difficult to reveal by measurements that are spatially averaged over many phase separated regions. The ability to simultaneously track the spatial and temporal evolution of such systems is essential to understanding mesoscopic processes during a phase transition. Using state-of-the-art time-resolved hard x-ray diffraction microscopy, we directly visualize the structural phase progression in a VO2 film upon photoexcitation. Following a homogenous in-plane optical excitation, the phase transformation is initiated at discrete sites and completed by the growth of one lattice structure into the other, instead of a simultaneous isotropic lattice symmetry change. The time-dependent x-ray diffraction spatial maps show that the in-plane phase progression in laser-superheated VO2 is via a displacive lattice transformation as a result of relaxation from an excited monoclinic phase into a rutile phase. The speed of the phase front progression is quantitatively measured, and is faster than the process driven by in-plane thermal diffusion but slower than the sound speed in VO2. The direct visualization of localized structural changes in the time domain opens a new avenue to study mesoscopic processes in driven systems.

  5. Study of x-ray emission enhancement via high contrast femtosecond laser interacting with solid foil

    International Nuclear Information System (INIS)

    Chen, Liming; Kando, Masaki; Bulanov, S.V.; Koga, James K.; Tajima, Toshiki; Xu M.H.; Yuan X.H.; Li Y.T.; Dong Q.L.; Zhang J.

    2007-01-01

    We studied the hard x-ray emission and the Kα x-ray conversion efficiency (η K ) produced by 60 fs high contrast frequency doubled Ti: sapphire laser pulse focused on Cu foil target. Cu Kα photon emission obtained with second harmonic laser pulse is more intense than the case of fundamental laser pulse. The Cu η K shows strong dependence on laser nonlinearly skewed pulse shape and reaches the maximum value 4x10 -4 with 100 fs negatively skewed pulse. It shows the electron spectrum shaping contribute to the increase of η K . (author)

  6. Lasers and laser applications. Imaging implosion dynamics: The x-ray pinhole/streak camera

    International Nuclear Information System (INIS)

    Attwood, D.T.

    1976-01-01

    A Livermore-developed x-ray-sensitive streak camera was combined with a unique x-ray pinhole camera to make dynamic photographs of laser-irradiated fusion target implosions. These photographs show x radiation emitted from the imploding shell during its 100-ps implosion; they are the first continuous observations of an imploding laser-driven fusion capsule. The diagnostic system has a time resolution of 15 ps and a spatial resolution of about 6 μm. Results agree very well with those predicted by our LASNEX calculations, confirming that the essential physics are correctly described in the code and providing further confidence in the soundness of this approach to inertial confinement fusion

  7. Static and time-resolved 10-1000 keV x-ray imaging detector options for NIF

    International Nuclear Information System (INIS)

    Landen, O.L.; Bell, P.M.; McDonald, J.W.; Park, H.-S.; Weber, F.; Moody, J.D.; Lowry, M.E.; Stewart, R.E.

    2004-01-01

    High energy (>10 keV) x-ray self-emission imaging and radiography will be essential components of many NIF high energy density physics experiments. In preparation for such experiments, we have evaluated the pros and cons of various static [x-ray film, bare charge-coupled device (CCD), and scintillator + CCD] and time-resolved (streaked and gated) 10-1000 keV detectors

  8. Studies of nanostructures using time-resolved x-ray excited optical luminescence*

    International Nuclear Information System (INIS)

    Rosenberg, R.A.; Shenoy, G.K.; Smita, S.; Burda, C.; Sham, T.K.

    2004-01-01

    Full text:The scientific community is currently investing a great deal of effort into understanding the physics and chemistry of nanoscale structures. Synchrotron radiation techniques are being used to study the physical, electronic, and magnetic structure of nanosystems, albeit at a relatively large size (greater than 30 nm). A major challenge facing researchers is finding methods that can probe structures of the smallest scale (less than 10 nm). Optical luminescence has been shown to be directly sensitive to structures in this size range due to quantum confinement phenomena. X-ray-excited optical luminescence (XEOL) provides the capability to chemically map the sites responsible for producing low-energy (1-6 eV) fluorescence. By taking advantage of the time structure of the x-ray pulses at the Advanced Photon Source (70 ps wide, 153 ns separation), it also possible to determine the dynamic behavior of the states involved in the luminescence. In this paper we will present results of time-resolved XEOL experiments on various nanostructures including porous silicon, silicon nanowires, and CdSe nanodots

  9. Spatially resolved synchrotron radiation induced X-ray fluorescence analyses of rare Rembrandt silverpoint drawings

    International Nuclear Information System (INIS)

    Reiche, I.; Radtke, M.; Berger, A.; Goerner, W.; Merchel, S.; Riesemeier, H.; Bevers, H.

    2006-01-01

    New analyses of a series of very rare silverpoint drawings that were executed by Rembrandt Harmensz. van Rijn (1606-1669) which are kept today in the Kupferstichkabinett (Museum of Prints and Drawings) of the State Museums of Berlin are reported here. Analysis of these drawings requires particular attention because the study has to be fully non-destructive and extremely sensitive. The metal alloy on the paper does not exceed some hundreds of μg/cm 2 . Therefore, synchrotron radiation induced X-ray fluorescence (SR-XRF) is - together with external micro-proton-induced X-ray emission - the only well-suited method for the analyses of metalpoint drawings. In some primary work, about 25 German and Flemish metalpoint drawings were investigated using spatially resolved SR-XRF analysis at the BAMline at BESSY. This study enlarges the existing French-German database of metalpoint drawings dating from the 15th and 16th centuries, as these Rembrandt drawings originate from the 17th century where this graphical technique was even rarer and already obsolete. It also illustrates how SR-XRF analysis can reinforce art historical assumptions on the dating of drawings and their connection. (orig.)

  10. Space resolved x-ray diffraction measurements of the supercooled state of polymers

    International Nuclear Information System (INIS)

    Asano, Tsutomu; Yoshida, Shinya; Nishida, Akira; Mina, M.F.

    2002-01-01

    In order to measure an ordering process of polymers, the supercooled state near the crystallizing surface was observed by a space resolved X-ray diffraction method at Photon Factory (PF). Using temperature slope crystallization, low density polyethylene and even-number paraffins were examined during crystallization from the melt state. The results indicate that polyethylene shows a sharp b-axis orientation where the lamellar normal and crystalline c-axis are perpendicular to the temperature slope. The crystalline lamellae are well-developed with lamellar thickness of 180 A. The supercooled melt state just above the crystallizing plane shows some diffraction in the small angle region without any crystalline reflection in the wide angle. This fact suggests that a long-range ordering (lamellar structure) appears prior to the short-range one (crystalline structure). The in-situ crystallizing surface was observed by an optical microscope connected to a TV system. The crystallizing surface of even-number paraffins moves to upwards in the temperature slope. In-situ X-ray measurements at PF revealed that the crystalline c-axis and lamellar normal of the even number paraffins are parallel to the temperature slope. From these results, the crystalline ordering and the surface movement of even number paraffins are explained using special nucleation mechanism including a screw dislocation. (author)

  11. Characterisation and application of a laser-based hard x-ray source

    International Nuclear Information System (INIS)

    Graetz, M.

    1998-11-01

    Hard X-rays are generated by focusing 110 fs laser pulses with intensities of about 1017 W/cm 2 onto solid metal targets. Characteristic properties of this X-ray source are the small source size, the short pulse duration and the high peak flux. The aim of the present work was to characterise this X-ray source and to demonstrate possible applications. A comparison with other X-ray sources and conventional imaging techniques is made. Characterising measurements were performed, including source size, emission spectrum, temporal behaviour, source stability and the influence of various laser parameters. The emission spectrum was measured using both energy-dispersive solid-state detectors and wavelength-dispersive crystal spectroscopy. The conversion efficiency from laser light to X-ray radiation was measured for different target materials. The laser ablation from different targets was studied. The feasibility of special imaging techniques, e.g. differential imaging and time-gated imaging, was investigated both theoretically and experimentally. Differential imaging allows for selective imaging of contrast agents, while time-gated imaging can reduce the influence of scattered radiation in X-ray imaging. Time-gated imaging was demonstrated in different imaging geometries, both for planar imaging and computed tomography imaging. Reasonable agreement between theoretically calculated values and experimental results was obtained

  12. Characterisation and application of a laser-based hard x-ray source

    Energy Technology Data Exchange (ETDEWEB)

    Graetz, M

    1998-11-01

    Hard X-rays are generated by focusing 110 fs laser pulses with intensities of about 1017 W/cm{sup 2} onto solid metal targets. Characteristic properties of this X-ray source are the small source size, the short pulse duration and the high peak flux. The aim of the present work was to characterise this X-ray source and to demonstrate possible applications. A comparison with other X-ray sources and conventional imaging techniques is made. Characterising measurements were performed, including source size, emission spectrum, temporal behaviour, source stability and the influence of various laser parameters. The emission spectrum was measured using both energy-dispersive solid-state detectors and wavelength-dispersive crystal spectroscopy. The conversion efficiency from laser light to X-ray radiation was measured for different target materials. The laser ablation from different targets was studied. The feasibility of special imaging techniques, e.g. differential imaging and time-gated imaging, was investigated both theoretically and experimentally. Differential imaging allows for selective imaging of contrast agents, while time-gated imaging can reduce the influence of scattered radiation in X-ray imaging. Time-gated imaging was demonstrated in different imaging geometries, both for planar imaging and computed tomography imaging. Reasonable agreement between theoretically calculated values and experimental results was obtained 120 refs, figs, tabs

  13. Circular dichroism measurements at an x-ray free-electron laser with polarization control

    Energy Technology Data Exchange (ETDEWEB)

    Hartmann, G.; Shevchuk, I.; Walter, P.; Viefhaus, J. [Deutsches Elektronen-Synchrotron, Notkestraße 85, 22607 Hamburg (Germany); Lindahl, A. O. [PULSE at Stanford, 2575 Sand Hill Road, Menlo Park, California 94025 (United States); Knie, A. [Institut für Physik, University of Kassel, Heinrich-Plett-Str. 40, 34132 Kassel (Germany); Hartmann, N.; Lutman, A. A.; MacArthur, J. P.; Glownia, J. M.; Helml, W.; Huang, Z.; Marinelli, A.; Nuhn, H.-D.; Moeller, S.; Coffee, R. N.; Ilchen, M., E-mail: markus.ilchen@xfel.eu [SLAC National Accelerator Laboratory, 2575 Sand Hill Road, Menlo Park, California 94025 (United States); Buck, J.; Galler, A.; Liu, J. [European XFEL GmbH, Albert-Einstein-Ring 19, 22761 Hamburg (Germany); and others

    2016-08-15

    A non-destructive diagnostic method for the characterization of circularly polarized, ultraintense, short wavelength free-electron laser (FEL) light is presented. The recently installed Delta undulator at the LCLS (Linac Coherent Light Source) at SLAC National Accelerator Laboratory (USA) was used as showcase for this diagnostic scheme. By applying a combined two-color, multi-photon experiment with polarization control, the degree of circular polarization of the Delta undulator has been determined. Towards this goal, an oriented electronic state in the continuum was created by non-resonant ionization of the O{sub 2} 1s core shell with circularly polarized FEL pulses at hν ≃ 700 eV. An also circularly polarized, highly intense UV laser pulse with hν ≃ 3.1 eV was temporally and spatially overlapped, causing the photoelectrons to redistribute into so-called sidebands that are energetically separated by the photon energy of the UV laser. By determining the circular dichroism of these redistributed electrons using angle resolving electron spectroscopy and modeling the results with the strong-field approximation, this scheme allows to unambiguously determine the absolute degree of circular polarization of any pulsed, ultraintense XUV or X-ray laser source.

  14. Circular dichroism measurements at an x-ray free-electron laser with polarization control

    Science.gov (United States)

    Hartmann, G.; Lindahl, A. O.; Knie, A.; Hartmann, N.; Lutman, A. A.; MacArthur, J. P.; Shevchuk, I.; Buck, J.; Galler, A.; Glownia, J. M.; Helml, W.; Huang, Z.; Kabachnik, N. M.; Kazansky, A. K.; Liu, J.; Marinelli, A.; Mazza, T.; Nuhn, H.-D.; Walter, P.; Viefhaus, J.; Meyer, M.; Moeller, S.; Coffee, R. N.; Ilchen, M.

    2016-08-01

    A non-destructive diagnostic method for the characterization of circularly polarized, ultraintense, short wavelength free-electron laser (FEL) light is presented. The recently installed Delta undulator at the LCLS (Linac Coherent Light Source) at SLAC National Accelerator Laboratory (USA) was used as showcase for this diagnostic scheme. By applying a combined two-color, multi-photon experiment with polarization control, the degree of circular polarization of the Delta undulator has been determined. Towards this goal, an oriented electronic state in the continuum was created by non-resonant ionization of the O2 1s core shell with circularly polarized FEL pulses at hν ≃ 700 eV. An also circularly polarized, highly intense UV laser pulse with hν ≃ 3.1 eV was temporally and spatially overlapped, causing the photoelectrons to redistribute into so-called sidebands that are energetically separated by the photon energy of the UV laser. By determining the circular dichroism of these redistributed electrons using angle resolving electron spectroscopy and modeling the results with the strong-field approximation, this scheme allows to unambiguously determine the absolute degree of circular polarization of any pulsed, ultraintense XUV or X-ray laser source.

  15. Modeling of collisional excited x-ray lasers using short pulse laser pumping

    Energy Technology Data Exchange (ETDEWEB)

    Sasaki, Akira; Moribayashi, Kengo; Utsumi, Takayuki; Tajima, Toshiki [Japan Atomic Energy Research Inst., Neyagawa, Osaka (Japan). Kansai Research Establishment

    1998-03-01

    A simple atomic kinetics model of electron collisional excited x-ray lasers has been developed. The model consists of a collisional radiative model using the average ion model (AIM) and a detailed term accounting (DTA) model of Ni-like Ta. An estimate of plasma condition to produce gain in Ni-like Ta ({lambda}=44A) is given. Use of the plasma confined in a cylinder is proposed to preform a uniform high density plasma from 1-D hydrodynamics calculations. (author)

  16. The x-ray laser as a tool for imaging plasmas

    International Nuclear Information System (INIS)

    Libby, S.B.; Da Silva, L.B.; Barbee, T.W. Jr.

    1995-07-01

    The x-ray laser is now being used at LLNL as a tool for measuring the behaviors of hot dense plasmas. In particular, we have used the 155 Angstrom yttrium laser to study transient plasmas by both radiography and moire deflectrometry. These techniques have been used to probe long scale length plasmas at electron densities exceeding 10 22 cm -3 . Recent advances in multilayer technology have made it possible to directly image ion densities in directly driven thin foils to an accuracy of 1--2 μm. In addition, we have constructed an x-ray laser Mach-Zehnder interferometer using multilayer beam-splitters. This interferometer yields direct 2D projections of electron densities in plasmas with micron spatial resolution. In addition, this interferometer can be used to measure spectral line shapes to high accuracy. Among the subject plasmas under study are laser irradiated planar targets, gold hohlraums, and x-ray lasers themselves

  17. Development of XUV-interferometry (155 angstrom) using a soft x-ray laser

    International Nuclear Information System (INIS)

    Da Silva, L.B.; Barbee, T.W.; Cauble, R.

    1995-01-01

    Over the past several years the authors have developed a variety of techniques for probing plasmas with x-ray lasers. These have included direct high resolution plasma imaging to quantify laser produced plasma uniformities and moire deflectometry to measure electron density profiles in one-dimension. Although these techniques have been valuable, a need existed for direct two dimensional measurements of electron densities in large high density plasmas. For this reason the authors have worked on developing a xuv interferometer compatible with the harsh environment of laser produced plasmas. This paper describes the design and presents some results showing excellent fringe visibility using the neon-like yttrium x-ray laser operating at 155 angstrom. The coherence properties of this x-ray laser source were measured using interferometry and are also discussed

  18. System for automatic x-ray-image analysis, measurement, and sorting of laser fusion targets

    International Nuclear Information System (INIS)

    Singleton, R.M.; Perkins, D.E.; Willenborg, D.L.

    1980-01-01

    This paper describes the Automatic X-Ray Image Analysis and Sorting (AXIAS) system which is designed to analyze and measure x-ray images of opaque hollow microspheres used as laser fusion targets. The x-ray images are first recorded on a high resolution film plate. The AXIAS system then digitizes and processes the images to accurately measure the target parameters and defects. The primary goals of the AXIAS system are: to provide extremely accurate and rapid measurements, to engineer a practical system for a routine production environment and to furnish the capability of automatically measuring an array of images for sorting and selection

  19. Multi-keV X-ray area source intensity at SGII laser facility

    Science.gov (United States)

    Wang, Rui-rong; An, Hong-hai; Xie, Zhi-yong; Wang, Wei

    2018-05-01

    Experiments for investigating the feasibility of multi-keV backlighters for several different metallic foil targets were performed at the Shenguang II (SGII) laser facility in China. Emission spectra in the energy range of 1.65-7.0 keV were measured with an elliptically bent crystal spectrometer, and the X-ray source size was measured with a pinhole camera. The X-ray intensity near 4.75 keV and the X-ray source size for titanium targets at different laser intensity irradiances were studied. By adjusting the total laser energy at a fixed focal spot size, laser intensity in the range of 1.5-5.0 × 1015 W/cm2, was achieved. The results show that the line emission intensity near 4.75 keV and the X-ray source size are dependent on the laser intensity and increase as the laser intensity increases. However, an observed "peak" in the X-ray intensity near 4.75 keV occurs at an irradiance of 4.0 × 1015 W/cm2. For the employed experimental conditions, it was confirmed that the laser intensity could play a significant role in the development of an efficient multi-keV X-ray source. The experimental results for titanium indicate that the production of a large (˜350 μm in diameter) intense backlighter source of multi-keV X-rays is feasible at the SGII facility.

  20. Photoinduced charge transfer in a transition metal complex investigated by time-resolved X-ray absorption fine structure spectroscopy. Setup and experiment

    International Nuclear Information System (INIS)

    Goeries, Dennis

    2015-02-01

    In the framework of this thesis the development of a time-resolved X-ray absorption spectroscopy experiment and its application to fac-Ir(ppy) 3 is described. Such experiments require a very stable setup in terms of spatial and temporal accuracy. Therefore, the stability properties of the present installation were investigated in detail and continuously improved, in particular the synchronization of the ultrashort pulse laser system to the storage ring as well as the spatial stability of both X-ray and laser beam. Experiments utilizing the laser pump and X-ray probe configuration were applied on the green phosphorescence emitter complex fac-Ir(ppy) 3 dissolved in dimethyl sulfoxide. Structural and electronic changes were triggered by photoexcitation of the metal-to-ligand charge transfer band with ultrashort laser pulses at a wavelength of 343 nm. The excited triplet state spectrum was extracted from the measured pump-probe X-ray absorption spectrum using an ionic approximation. The results con rm the anticipated metal-to-ligand charge transfer as shown by an ionization potential shift of the iridium atom. The symmetry of the complex was found to be pseudo-octahedral. This allowed the first experimental determination of the bond length of fac-Ir(ppy) 3 in an octahedral approximation and revealed a decrease of bond length of the first coordination shell in the triplet state. The first and second-order decay kinetics of the triplet state were investigated in a combination of X-ray and laser based experiments and revealed self-quenching as well as triplet-triplet annihilation rate constants.

  1. Achieving few-femtosecond time-sorting at hard X-ray free-electron lasers

    Science.gov (United States)

    Harmand, M.; Coffee, R.; Bionta, M. R.; Chollet, M.; French, D.; Zhu, D.; Fritz, D. M.; Lemke, H. T.; Medvedev, N.; Ziaja, B.; Toleikis, S.; Cammarata, M.

    2013-03-01

    Recently, few-femtosecond pulses have become available at hard X-ray free-electron lasers. Coupled with the available sub-10 fs optical pulses, investigations into few-femtosecond dynamics are not far off. However, achieving sufficient synchronization between optical lasers and X-ray pulses continues to be challenging. We report a `measure-and-sort' approach, which achieves sub-10 fs root-mean-squared (r.m.s.) error measurement at hard X-ray FELs, far beyond the 100-200 fs r.m.s. jitter limitations. This timing diagnostic, now routinely available at the Linac Coherent Light Source (LCLS), is based on ultrafast free-carrier generation in optically transparent materials. Correlation between two independent measurements enables unambiguous demonstration of ~6 fs r.m.s. error in reporting the optical/X-ray delay, with single shot error suggesting the possibility of reaching few-femtosecond resolution.

  2. Two electron response to an intense x-ray free electron laser pulse

    International Nuclear Information System (INIS)

    Moore, L R; Parker, J S; Meharg, K J; Armstrong, G S J; Taylor, K T

    2009-01-01

    New x-ray free electron lasers (FELs) promise an ultra-fast ultra-intense regime in which new physical phenomena, such as double core hole formation in at atom, should become directly observable. Ahead of x-ray FEL experiments, an initial key task is to theoretically explore such fundamental laser-atom interactions and processes. To study the response of a two-electron positive ion to an intense x-ray FEL pulse, our theoretical approach is a direct numerical integration, incorporating non-dipole Hamiltonian terms, of the full six-dimensional time-dependent Schroedinger equation. We present probabilities of double K-shell ionization in the two-electron positive ions Ne 8+ and Ar 16+ exposed to x-ray FEL pulses with frequencies in the range 50 au to 300 au and intensities in the range 10 17 to 10 22 W/cm 2 .

  3. Two electron response to an intense x-ray free electron laser pulse

    Energy Technology Data Exchange (ETDEWEB)

    Moore, L R; Parker, J S; Meharg, K J; Armstrong, G S J; Taylor, K T, E-mail: l.moore@qub.ac.u [DAMTP, David Bates Building, Queen' s University Belfast, Belfast, BT7 1NN (United Kingdom)

    2009-11-01

    New x-ray free electron lasers (FELs) promise an ultra-fast ultra-intense regime in which new physical phenomena, such as double core hole formation in at atom, should become directly observable. Ahead of x-ray FEL experiments, an initial key task is to theoretically explore such fundamental laser-atom interactions and processes. To study the response of a two-electron positive ion to an intense x-ray FEL pulse, our theoretical approach is a direct numerical integration, incorporating non-dipole Hamiltonian terms, of the full six-dimensional time-dependent Schroedinger equation. We present probabilities of double K-shell ionization in the two-electron positive ions Ne{sup 8+} and Ar{sup 16+} exposed to x-ray FEL pulses with frequencies in the range 50 au to 300 au and intensities in the range 10{sup 17} to 10{sup 22} W/cm{sup 2}.

  4. Fabrication of polycrystalline diamond refractive X-ray lens by femtosecond laser processing

    Energy Technology Data Exchange (ETDEWEB)

    Kononenko, T.V.; Ralchenko, V.G.; Ashkinazi, E.E.; Konov, V.I. [General Physics Institute of Russian Academy of Sciences, Moscow (Russian Federation); National Research Nuclear University ' ' MEPhI' ' , Moscow (Russian Federation); Polikarpov, M.; Ershov, P. [Immanuel Kant Baltic Federal University, Functional Nanomaterials, Kaliningrad (Russian Federation); Kuznetsov, S.; Yunkin, V. [Institute of Microelectronics Technology RAS, Chernogolovka, Moscow region (Russian Federation); Snigireva, I. [European Synchrotron Radiation Facility, Grenoble (France)

    2016-03-15

    X-ray planar compound refractive lenses were fabricated from a polycrystalline diamond plate grown by chemical vapor deposition, by precise through cutting with femtosecond laser pulses. The lens geometry and the surface morphology were investigated with optical and scanning electron microscopy, while the material structure modification was analyzed by Raman spectroscopy. The results of the preliminary lens test at 9.25-keV X-rays are presented. (orig.)

  5. Fabrication of polycrystalline diamond refractive X-ray lens by femtosecond laser processing

    International Nuclear Information System (INIS)

    Kononenko, T.V.; Ralchenko, V.G.; Ashkinazi, E.E.; Konov, V.I.; Polikarpov, M.; Ershov, P.; Kuznetsov, S.; Yunkin, V.; Snigireva, I.

    2016-01-01

    X-ray planar compound refractive lenses were fabricated from a polycrystalline diamond plate grown by chemical vapor deposition, by precise through cutting with femtosecond laser pulses. The lens geometry and the surface morphology were investigated with optical and scanning electron microscopy, while the material structure modification was analyzed by Raman spectroscopy. The results of the preliminary lens test at 9.25-keV X-rays are presented. (orig.)

  6. Angle-resolved X-ray fluorescence spectrometry using synchrotron radiation at ELSA

    International Nuclear Information System (INIS)

    Schmitt, W.; Rothe, J.; Hormes, J.; Gries, W.H.

    1994-01-01

    Measurements on the centroid depth of ion-implanted phosphorus-in-silicon specimen by the method of angle-resolved, self-ratio X-ray fluorescence spectrometry (AR/SR/XFS) have been carried out using 'white' synchrotron radiation (SR). The measurements were performed using a modified wavelength-dispersive fluorescence spectrometer. Problems due to the use of SR, like carbonaceous specimen contamination and sample heating were overcome by flooding the specimen chamber with helium and by pre-absorbing the non-exciting parts of the incident SR with suitable filters, respectively. The decaying primary intensity was monitored by measuring the compensation current of the photoelectrons emitted from a tungsten wire stretched across the primary beam. Results have been obtained for specimen with dose density levels of 10 16 cm -2 and 3x10 15 cm -2 . (orig.)

  7. Direct Observation of Insulin Association Dynamics with Time-Resolved X-ray Scattering

    Energy Technology Data Exchange (ETDEWEB)

    Rimmerman, Dolev [Department; Leshchev, Denis [Department; Hsu, Darren J. [Department; Hong, Jiyun [Department; Kosheleva, Irina [Center; Chen, Lin X. [Department; Chemical

    2017-09-05

    Biological functions frequently require protein-protein interactions that involve secondary and tertiary structural perturbation. Here we study protein-protein dissociation and reassociation dynamics in insulin, a model system for protein oligomerization. Insulin dimer dissociation into monomers was induced by a nanosecond temperature-jump (T-jump) of ~8 °C in aqueous solution, and the resulting protein and solvent dynamics were tracked by time-resolved X-ray solution scattering (TRXSS) on time scales of 10 ns to 100 ms. The protein scattering signals revealed the formation of five distinguishable transient species during the association process that deviate from simple two state kinetics. Our results show that the combination of T-jump pump coupled to TRXSS probe allows for direct tracking of structural dynamics in nonphotoactive proteins.

  8. Structure-activity relationships of heterogeneous catalysts from time-resolved X-ray absorption spectroscopy

    International Nuclear Information System (INIS)

    Ressler, T.; Jentoft, R.E.; Wienold, J.; Girgsdies, F.; Neisius, T.; Timpe, O.

    2003-01-01

    Knowing the composition and the evolution of the bulk structure of a heterogeneous catalyst under working conditions (in situ) is a pre-requisite for understanding structure-activity relationships. X-ray absorption spectroscopy can be employed to study a catalytically active material in situ. In addition to steady-state investigations, the technique permits experiments with a time-resolution in the sub-second range to elucidate the solid-state kinetics of the reactions involved. Combined with mass spectrometry, the evolution of the short-range order structure of a heterogeneous catalyst, the average valence of the constituent metals, and the phase composition can be obtained. Here we present results obtained from time-resolved studies on the reduction of MoO 3 in propene and in propene and oxygen

  9. Excitation-resolved cone-beam x-ray luminescence tomography.

    Science.gov (United States)

    Liu, Xin; Liao, Qimei; Wang, Hongkai; Yan, Zhuangzhi

    2015-07-01

    Cone-beam x-ray luminescence computed tomography (CB-XLCT), as an emerging imaging technique, plays an important role in in vivo small animal imaging studies. However, CB-XLCT suffers from low-spatial resolution due to the ill-posed nature of reconstruction. We improve the imaging performance of CB-XLCT by using a multiband excitation-resolved imaging scheme combined with principal component analysis. To evaluate the performance of the proposed method, the physical phantom experiment is performed with a custom-made XLCT/XCT imaging system. The experimental results validate the feasibility of the method, where two adjacent nanophosphors (with an edge-to-edge distance of 2.4 mm) can be located.

  10. Demonstration of Laser Plasma X-Ray Source with X-Ray Collimator Final Report CRADA No. TC-1564-99

    Energy Technology Data Exchange (ETDEWEB)

    Lane, S. M. [Lawrence Livermore National Lab. (LLNL), Livermore, CA (United States); Forber, R. A. [Lawrence Livermore National Lab. (LLNL), Livermore, CA (United States)

    2017-09-28

    This collaborative effort between the University of California, Lawrence Livermore National Laboratory (LLNL) and JMAR Research, Inc. (JRI), was to demonstrate that LLNL x-ray collimators can effectively increase the wafer throughput of JRI's laser based x-ray lithography systems. The technical objectives were expected to be achieved by completion of the following tasks, which are separated into two task lists by funding source. The organization (LLNL or JMAR) having primary responsibility is given parenthetically for each task.

  11. X-ray absorption in characterization of laser fusion targets

    International Nuclear Information System (INIS)

    Clement, X.; Coudeville, A.; Eyharts, P.; Perrine, J.P.; Rouillard, R.

    1982-11-01

    Many plastic or metal coated targets are opaque, so their thickness and thickness uniformity cannot be obtained by optical means. Therefore, we have built and tested a new system using monochromatic X-ray absorption measurements. This system is also able to perform non-destructive measurements of argon fill pressure in glass microballoons. The X-ray source is a diffraction tube with a chromium target and fine focus (0.4 x 0.8 mm 2 ). Since monochromatic calculations are involved in this method, we use electronic discrimination to isolate the chromium Kα line (5.4 keV) from the bremsstrahlung spectrum. The detectors are xenon-filled proportional counters. The system is composed of two beams (10 μm in diameter), one used as a reference and the other as the measurement arm. A PET desk computer is coupled ot the experiment. We achieved a precision better than 10% for gold layers in the range of 0.1 to 1 μm, and better than 20% for argon pressures in the range of 5 - 13 bars

  12. Soft x-ray generation in gases with an ultrashort pulse laser

    Energy Technology Data Exchange (ETDEWEB)

    Ditmire, Todd Raymond [Univ. of California, Davis, CA (United States)

    1996-01-08

    An experimental investigation of soft x-ray production resulting from the interaction of intense near infra-red laser radiation with gases is presented in this thesis. Specifically, soft x-ray generation through high order harmonic generation or exploiting intense inverse bremsstrahlung heating is examined. Most of these studies are conducted with femtosecond, terawatt class Cr:LiSrAlF6 (LiSAF) laser, though results derived from studies with other laser systems are presented as well. The majority of this work is devoted to experimental investigations, however, theoretical and computational models are developed to interpret the data. These studies are motivated by the possibility of utilizing the physics of intense laser/matter interactions as a potential compact source of bright x-rays. Consequently, the thrust of many of the experiments conducted is aimed at characterizing the x-rays produced for possible use in applications. In general, the studies of this manuscript fall into three categories. First, a unique 130 fs, 8 TW laser that is based on chirped pulse amplification, is described, and its performance is evaluated. The generation of x-rays through high order harmonics is then discussed with emphasis on characterizing and optimizing harmonic generation. Finally, the generation of strong, incoherent x-ray radiation by the intense irradiation of large (>1,000 atom) clusters in gas jets, is explored. The physics of laser energy absorption by clusters illuminated with intensities of 1015 to 1017 W/cm2 is considered in detail. X-ray spectroscopy of the hot plasmas that result from the irradiation of the clusters is conducted, and energy transport and kinetics issues in these plasmas are discussed.

  13. A final report to the Laboratory Directed Research and Development committee on Project 93-ERP-075: ''X-ray laser propagation and coherence: Diagnosing fast-evolving, high-density laser plasmas using X-ray lasers''

    International Nuclear Information System (INIS)

    Wan, A.S.; Cauble, R.; Da Silva, L.B.; Libby, S.B.; Moreno, J.C.

    1996-02-01

    This report summarizes the major accomplishments of this three-year Laboratory Directed Research and Development (LDRD) Exploratory Research Project (ERP) entitled ''X-ray Laser Propagation and Coherence: Diagnosing Fast-evolving, High-density Laser Plasmas Using X-ray Lasers,'' tracking code 93-ERP-075. The most significant accomplishment of this project is the demonstration of a new laser plasma diagnostic: a soft x-ray Mach-Zehnder interferometer using a neonlike yttrium x-ray laser at 155 angstrom as the probe source. Detailed comparisons of absolute two-dimensional electron density profiles obtained from soft x-ray laser interferograms and profiles obtained from radiation hydrodynamics codes, such as LASNEX, will allow us to validate and benchmark complex numerical models used to study the physics of laser-plasma interactions. Thus the development of soft x-ray interferometry technique provides a mechanism to probe the deficiencies of the numerical models and is an important tool for, the high-energy density physics and science-based stockpile stewardship programs. The authors have used the soft x-ray interferometer to study a number of high-density, fast evolving, laser-produced plasmas, such as the dynamics of exploding foils and colliding plasmas. They are pursuing the application of the soft x-ray interferometer to study ICF-relevant plasmas, such as capsules and hohlraums, on the Nova 10-beam facility. They have also studied the development of enhanced-coherence, shorter-pulse-duration, and high-brightness x-ray lasers. The utilization of improved x-ray laser sources can ultimately enable them to obtain three-dimensional holographic images of laser-produced plasmas

  14. Efficient soft x-ray generation in short wavelength laser produced plasmas

    International Nuclear Information System (INIS)

    Mochizuki, T.; Yamanaka, C.

    1987-01-01

    Intense x-ray generation in 1.053, 0.53, 0.26 μm laser-produced plasma has been investigated in the photon energy range of 0.1 to 3keV. The x-ray spectrum is found to have several humps which move to the higher energy side as the atomic number of the target increases. This atomic dependence is explained by a semi-Moseley's law and allows us to predict a target material most suitable for generating the photons of desired energies. Conversion efficiencies of 1.5 -- 3keV x-rays are obtained also as a function of laser wavelength at the intensity of 10/sup 13/W/cm/sup 2/. The conversion efficiency of keV x rays has been enhanced by a factor of 2 -- 3 with a controlled prepulse laser. From the semi-Moseley's law we find that cryogenic targets using either Xe or Kr in a liquid or solid phase may be most useful for a number of applications because they radiate 1 -- 3 keV x rays efficiently and never deposit on the x-ray optical components and the objects to be exposed

  15. [Experimental investigation of laser plasma soft X-ray source with gas target].

    Science.gov (United States)

    Ni, Qi-liang; Gong, Yan; Lin, Jing-quan; Chen, Bo; Cao, Jian-lin

    2003-02-01

    This paper describes a debris-free laser plasma soft X-ray source with a gas target, which has high operating frequency and can produce strong soft X-ray radiation. The valve of this light source is drived by a piezoelectrical ceramic whose operating frequency is up to 400 Hz. In comparison with laser plasma soft X-ray sources using metal target, the light source is debris-free. And it has higher operating frequency than gas target soft X-ray sources whose nozzle is controlled by a solenoid valve. A channel electron multiplier (CEM) operating in analog mode is used to detect the soft X-ray generated by the laser plasma source, and the CEM's output is fed to to a charge-sensitive preamplifier for further amplification purpose. Output charges from the CEM are proportional to the amplitude of the preamplifier's output voltage. Spectra of CO2, Xe and Kr at 8-14 nm wavelength which can be used for soft X-ray projection lithography are measured. The spectrum for CO2 consists of separate spectral lines originate mainly from the transitions in Li-like and Be-like ions. The Xe spectrum originating mainly from 4d-5f, 4d-4f, 4d-6p and 4d-5p transitions in multiply charged xenon ions. The spectrum for Kr consists of separate spectral lines and continuous broad spectra originating mainly from the transitions in Cu-, Ni-, Co- and Fe-like ions.

  16. In situ laser heating and radial synchrotron X-ray diffraction ina diamond anvil cell

    Energy Technology Data Exchange (ETDEWEB)

    Kunz, Martin; Caldwell, Wendel A.; Miyagi, Lowell; Wenk,Hans-Rudolf

    2007-06-29

    We report a first combination of diamond anvil cell radialx-ray diffraction with in situ laser heating. The laser-heating setup ofALS beamline 12.2.2 was modified to allow one-sided heating of a samplein a diamond anvil cell with an 80 W yttrium lithium fluoride laser whileprobing the sample with radial x-ray diffraction. The diamond anvil cellis placed with its compressional axis vertical, and perpendicular to thebeam. The laser beam is focused onto the sample from the top while thesample is probed with hard x-rays through an x-ray transparentboron-epoxy gasket. The temperature response of preferred orientation of(Fe,Mg)O is probed as a test experiment. Recrystallization was observedabove 1500 K, accompanied by a decrease in stress.

  17. Studies of momentum transfer and X-ray spectra in a laser-produced plasma

    International Nuclear Information System (INIS)

    Leroy, Pierre

    Studies of momentum transfer from a ballistic pendulum appear to give satisfactory results for absorbed laser energies in excess of 200 mJ i.e. for fluxes in the 3.10 10 to 3.10 12 W.cm -2 range. A hard X-ray component attributed to fast electrons was revealed by an X-ray spectrometer with a PM system of greater sensitivity than PIN diodes. The laser energy is however too weak to enable studies to be conducted as a function of laser flux or measurements to be performed on targets of low Z [fr

  18. Measurements of laser-hole boring into overdense plasmas using x-ray laser refractometry (invited)

    International Nuclear Information System (INIS)

    Kodama, R.; Takahashi, K.; Tanaka, K.A.; Kato, Y.; Murai, K.; Weber, F.; Barbee, T.W.; DaSilva, L.B.

    1999-01-01

    We developed a 19.6 nm laser x-ray laser grid-image refractometer (XRL-GIR) to diagnose laser-hole boring into overdense plasmas. The XRL-GIR was optimized to measure two-dimensional electron density perturbation on a scale of a few tens of μm in underdense plasmas. Electron density profiles of laser-produced plasmas were obtained for 10 20 - 10 22 cm -3 with the XRL-GIR and for 10 19 - 10 20 cm -3 from an ultraviolet interferometer, the profiles of which were compared with those from hydrodynamic simulation. By using this XRL-GIR, we directly observed laser channeling into overdense plasmas accompanied by a bow shock wave showing a Mach cone ascribed to supersonic propagation of the channel front. copyright 1999 American Institute of Physics

  19. Development of soft x-ray time-resolved photoemission spectroscopy system with a two-dimensional angle-resolved time-of-flight analyzer at SPring-8 BL07LSU

    Energy Technology Data Exchange (ETDEWEB)

    Ogawa, Manami; Yamamoto, Susumu; Nakamura, Fumitaka; Yukawa, Ryu; Fukushima, Akiko; Harasawa, Ayumi; Kakizaki, Akito; Matsuda, Iwao [Institute for Solid State Physics, University of Tokyo, 5-1-5 Kashiwanoha, Chiba 277-8581 (Japan); Kousa, Yuka; Kondoh, Hiroshi [Department of Chemistry, Keio University, Yokohama 223-8522 (Japan); Tanaka, Yoshihito [RIKEN/SPring-8 Center, 1-1-1, Kouto, Sayo-cho, Sayo-gun, Hyogo 679-5148 (Japan)

    2012-02-15

    We have developed a soft x-ray time-resolved photoemission spectroscopy system using synchrotron radiation (SR) at SPring-8 BL07LSU and an ultrashort pulse laser system. Two-dimensional angle-resolved measurements were performed with a time-of-flight-type analyzer. The photoemission spectroscopy system is synchronized to light pulses of SR and laser using a time control unit. The performance of the instrument is demonstrated by mapping the band structure of a Si(111) crystal over the surface Brillouin zones and observing relaxation of the surface photo-voltage effect using the pump (laser) and probe (SR) method.

  20. From laser-plasma accelerators to femtosecond X-ray sources: study, development and applications

    International Nuclear Information System (INIS)

    Corde, S.

    2012-01-01

    During the relativistic interaction between a short and intense laser pulse and an underdense plasma, electrons can be injected and accelerated up to hundreds of MeV in an accelerating structure formed in the wake of the pulse: this is the so-called laser-plasma accelerator. One of the major perspectives for laser-plasma accelerators resides in the realization of compact sources of femtosecond x-ray beams. In this thesis, two x-ray sources was studied and developed. The betatron radiation, intrinsic to laser-plasma accelerators, comes from the transverse oscillations of electrons during their acceleration. Its characterization by photon counting revealed an x-ray beam containing 10"9 photons, with energies extending above 10 keV. We also developed an all-optical Compton source producing photons with energies up to hundreds of keV, based on the collision between a photon beam and an electron beam. The potential of these x-ray sources was highlighted by the realization of single shot phase contrast imaging of a biological sample. Then, we showed that the betatron x-ray radiation can be a powerful tool to study the physics of laser-plasma acceleration. We demonstrated the possibility to map the x-ray emission region, which gives a unique insight into the interaction, permitting us for example to locate the region where electrons are injected. The x-ray angular and spectral properties allow us to gain information on the transverse dynamics of electrons during their acceleration. (author)

  1. Optimising hard X-ray generation from laser-produced plasmas

    International Nuclear Information System (INIS)

    Lindheimer, C.

    1995-04-01

    The aim of this work is to increase the X-ray yield for a laser produced plasma by optimising the focusing conditions and temporal shape of the laser pulses. The focusing conditions are improved by introducing a control system that secures the laser target surface to exact focus within a range of a few micrometers, allowing continuously high laser intensity for plasma generation. The temporal shape of the laser pulses is changed by introducing a saturable absorber in the laser beam. The laser produces a substantial pre-pulse that heats and expands the target material prior to main pulse arrival. The saturable absorber can increase the main pulse/pre-pulse ratio of the laser pulse up to four orders of magnitude and consequently reduce expansion of the target material before the main pulse. The belief is that an increase in target density at the time of main pulse arrival will change the energy distribution of the X-rays, towards a more efficient X-ray production in the hard X-ray region. This report and the work connected to it, includes the preliminary measurements and results for these improvements. 17 refs

  2. Near field imaging of transient collisional excitation x-ray laser

    International Nuclear Information System (INIS)

    Tanaka, Momoko; Kado, Masataka; Hasegawa, Noboru; Kawachi, Tetsuya; Sukegawa, Kouta; Lu, Peixiang; Nagashima, Akira; Kato, Yoshiaki

    2001-01-01

    We observed the spatial profile of the transient collisional excitation Ni-like Ag laser (λ=13.9 nm) for various plasma lengths using the near field imaging method. The gain coefficient of the x-ray laser was estimated as 24 cm -1 . The gain region was a 50 μm crescent shape and included localized high gain areas. (author)

  3. Characterization of collisionally pumped optical-field-ionization soft X-ray lasers

    Czech Academy of Sciences Publication Activity Database

    Mocek, Tomáš; Sebban, S.; Bettaibi, I.; Upcraft, L. M.; Balcou, P.; Breger, P.; Zeitoun, P.; Le Pape, S.; Ros, D.; Klisnick, A.; Carillon, A.; Jamelot, G.; Rus, Bedřich; Wyart, J. F.

    2004-01-01

    Roč. 78, - (2004), s. 939-944 ISSN 0946-2171 Grant - others:HPRI(XE) 199900086 Institutional research plan: CEZ:AV0Z1010921 Keywords : X-ray lasers * optical-field-ionization * collisional excitation Subject RIV: BH - Optics, Masers, Lasers Impact factor: 2.215, year: 2004

  4. Asymmetrically cut crystal pair as x-ray magnifier for imaging at high intensity laser facilities

    Energy Technology Data Exchange (ETDEWEB)

    Szabo, C. I.; Feldman, U. [Artep Inc., 2922 Excelsior Spring Circle, Ellicott City, Maryland 21042 (United States); Seely, J. F. [Space Science Division, Naval Research Laboratory, Washington, DC 20375-5352 (United States); Curry, J. J.; Hudson, L. T.; Henins, A. [National Institute of Standards and Technology, Gaithersburg, Maryland 20899 (United States)

    2010-10-15

    The potential of an x-ray magnifier prepared from a pair of asymmetrically cut crystals is studied to explore high energy x-ray imaging capabilities at high intensity laser facilities. OMEGA-EP and NIF when irradiating mid and high Z targets can be a source of high-energy x-rays whose production mechanisms and use as backlighters are a subject of active research. This paper studies the properties and potential of existing asymmetric cut crystal pairs from the National Institute of Standards and Technology (NIST) built in a new enclosure for imaging x-ray sources. The technique of the x-ray magnifier has been described previously. This new approach is aimed to find a design that could be used at laser facilities by magnifying the x-ray source into a screen far away from the target chamber center, with fixed magnification defined by the crystals' lattice spacing and the asymmetry angles. The magnified image is monochromatic and the imaging wavelength is set by crystal asymmetry and incidence angles. First laboratory results are presented and discussed.

  5. A development of laser-plasma-based soft x-ray microscope system

    Energy Technology Data Exchange (ETDEWEB)

    Nam, Ki Yong; Kim, Kyong Woo; Kim, Kyu Gyeom; Kwon, Young Man; Yoon, Kwon Ha [X-ray Microscopy Research Center, Wonkwang University, Iksan (Korea, Republic of)

    2003-07-01

    Soft x-ray nano-imaging microscopy system for biomedical application with a high resolution about 50 nm has been designed and described, and its integrated techniques also have been studied. The system is mainly composed of soft x-ray generation system, nano-scaled control system, x-ray optical device like a condenser or object mirror, a CCD camera coupled with multichannel plate (MCP) and vacuum system. In the system, soft x-ray is generated from the laser-based plasma by focusing Nd:YAG laser beam on tantalum (Ta) target. In an x-ray optical system, a wolter mirror has been considering condensing the x-ray beam on a biological specimen and zone plate was adapted as an object mirror. A Si{sub 3}N{sub 4} was used as specimen holder for keeping a biological sample alive in atmosphere conditions. A back-illuminated-CCD camera coupled with multichannel plate was determined to set up.

  6. Single-shot beam-position monitor for x-ray free electron laser

    Science.gov (United States)

    Tono, Kensuke; Kudo, Togo; Yabashi, Makina; Tachibana, Takeshi; Feng, Yiping; Fritz, David; Hastings, Jerome; Ishikawa, Tetsuya

    2011-02-01

    We have developed an x-ray beam-position monitor for detecting the radiation properties of an x-ray free electron laser (FEL). It is composed of four PIN photodiodes that detect backscattered x-rays from a semitransparent diamond film placed in the beam path. The signal intensities from the photodiodes are used to compute the beam intensity and position. A proof-of-principle experiment at a synchrotron light source revealed that the error in the beam position is reduced to below 7 μm by using a nanocrystal diamond film prepared by plasma-enhanced chemical vapor deposition. Owing to high dose tolerance and transparency of the diamond film, the monitor is suitable for routine diagnostics of extremely intense x-ray pulses from the FEL.

  7. Statistical and coherence properties of radiation from X-ray free electron lasers

    International Nuclear Information System (INIS)

    Saldin, E.L.; Schneidmiller, E.A.; Yurkov, M.V.

    2009-12-01

    We describe statistical and coherence properties of the radiation from X-ray free electron lasers (XFEL). It is shown that the X-ray FEL radiation before saturation is described with gaussian statistics. Particularly important is the case of the optimized X-ray FEL, studied in detail. Applying similarity techniques to the results of numerical simulations allowed us to find universal scaling relations for the main characteristics of an X-ray FEL operating in the saturation regime: efficiency, coherence time and degree of transverse coherence. We find that with an appropriate normalization of these quantities, they are functions of only the ratio of the geometrical emittance of the electron beam to the radiation wavelength. Statistical and coherence properties of the higher harmonics of the radiation are highlighted as well. (orig.)

  8. Statistical and coherence properties of radiation from X-ray free electron lasers

    Energy Technology Data Exchange (ETDEWEB)

    Saldin, E L; Schneidmiller, E A; Yurkov, M V

    2009-12-15

    We describe statistical and coherence properties of the radiation from X-ray free electron lasers (XFEL). It is shown that the X-ray FEL radiation before saturation is described with gaussian statistics. Particularly important is the case of the optimized X-ray FEL, studied in detail. Applying similarity techniques to the results of numerical simulations allowed us to find universal scaling relations for the main characteristics of an X-ray FEL operating in the saturation regime: efficiency, coherence time and degree of transverse coherence. We find that with an appropriate normalization of these quantities, they are functions of only the ratio of the geometrical emittance of the electron beam to the radiation wavelength. Statistical and coherence properties of the higher harmonics of the radiation are highlighted as well. (orig.)

  9. Sub-keV, subnanosecond measurements of x-ray spectra from laser-produced plasmas

    International Nuclear Information System (INIS)

    Kornblum, H.N.; Koppel, L.N.; Slivinsky, V.W.; Glaros, S.S.; Ahlstrom, H.G.; Larsen, J.T.

    1977-01-01

    As part of the effort to extend our x-ray diagnostic capabilities, we have made x-ray spectral measurements of laser-produced plasmas for photon energies down to 100 eV with a time response of 0.5 nsec. Fast, windowless x-ray diodes were used in conjunction with critical angle reflecting mirrors and thin filters for energy definition for two channels, 300 to 600 eV and 800 to 1300 eV. A third channel, using only an x-ray diode and filter, provided spectral information in the 100 to 300 eV region. Results from exploding pusher targets will be presented and compared with those of other diagnostic techniques and Lasnex calculations. Future expansion and modifications of the present system will be discussed

  10. Two-dimensional time-resolved X-ray diffraction study of directional solidification in steels

    International Nuclear Information System (INIS)

    Yonemura, Mitsuharu

    2009-01-01

    Full text: The high intensity heat source used for fusion welding creates steep thermal gradients of 100 degree C/s from 1800 degree Celsius. Further, the influence of a preferred orientation is serious for observation of a directional solidification that follows the dendrite growth along the direction toward the moving heat source. Therefore, we observed the rapid solidification of weld metal at a time resolution of 0.01∼0.1seconds by the Two-Dimensional Time-Resolved X-ray Diffraction (2DTRXRD) system for real welding. The diffraction ring was dynamically observed by 2DTRXRD during arc-passing over the irradiation area of X-ray with synchrotron energy of 18 KeV. The arc power output was 10 V - 150 A, and a scan speed of the arc was 1.0 mm/s. The temperature rise of instruments was suppressed by the water-cooled copper plate under the sample. Further, the temperature distribution of the weld metal was measured by the thermocouple and related to the diffraction patterns. Consequently, solidification and solid phase transformation of low carbon steels and stainless steels were observed during rapid cooling by 2DTRXRD. In the low-carbon steel, the microstructure is formed in the 2 step process; (i) formation of crystallites and (ii) increase of crystallinity. In the stainless steel, the irregular interface layer of σ/y in the quenched metal after solidification is expected that it is easy for dendrites to move at the lower temperature. In the carbide precipitation stainless steel, it is easy for NbC to grow on σ phase with a little under cooling. Further, a mist-like pattern, which differs from the halo-pattern, in the fusion zone gave some indication of the possibilities to observe the nucleation and the early solidification by 2DTRXRD. (author)

  11. Phase-Resolved Spectroscopy of the Low-Mass X-ray Binary V801 Ara

    Science.gov (United States)

    Brauer, Kaley; Vrtilek, Saeqa Dil; Peris, Charith; McCollough, Michael

    2018-06-01

    We present phase-resolved optical spectra of the low mass X-ray binary system V801 Ara. The spectra, obtained in 2014 with IMACS on the Magellan/Baade telescope at Las Campanas Observatory, cover the full binary orbit of 3.8 hours. They contain strong emission features allowing us to map the emission of Hα, Hβ, He II λ4686, and the Bowen blend at λ4640. The radial velocity curves of the Bowen blend shows significantly stronger modulation at the orbital period than Hα as expected for the former originating on the secondary with the latter consistent with emission dominated by the disk. Our tomograms of Hα and Hβ are the most detailed studies of these lines for V801 to date and they clearly detect the accretion disk. The Hβ emission extends to higher velocities than Hα, suggesting emission from closer to the neutron star and differentiating temperature variance in the accretion disk for the first time. The center of the accretion disk appears offset from the center-of-mass of the neutron star as has been seen in several other X-ray binaries. This is often interpreted to imply disk eccentricity. Our tomograms do not show strong evidence for a hot spot at the point where the accretion stream hits the disk. This could imply a reduced accretion rate or could be due to the spot being drowned out by bright accretion flow around it. There is enhanced emission further along the disk, however, which implies gas stream interaction downstream of the hot spot.

  12. Overview of the program on soft x-ray lasers and their applications at Princeton

    International Nuclear Information System (INIS)

    Suckewer, S.; Ilcisin, K.; Princeton Univ., NJ

    1991-05-01

    In the last several years, rapid progress in the development of soft x-ray lasers (SXL) has been observed at a number of laboratories worldwide. Although SXLs are very ''young'' devices they have already been used for microscopy and holography, and new ideas emerging for broader application of SXLs to microscopy, holography and lithography. This paper describes the work at Princeton University on the development of a soft x-ray imaging transmission microscopy using a SXL as a radiation source and work on the development of a novel soft x-ray reflection microscope and its application to biological cell studies and lithography. Progress in the development of a photopumped VUV laser (60 nm), and programs for the development of a small scale SXL and for the application of a powerful subpicosecond KrF laser system are also discussed. 35 refs., 9 figs., 1 tab

  13. K-edge x-ray-absorption spectroscopy of laser-generated Kr+ and Kr2+

    International Nuclear Information System (INIS)

    Southworth, S. H.; Arms, D. A.; Dufresne, E. M.; Dunford, R. W.; Ederer, D. L.; Hoehr, C.; Kanter, E. P.; Kraessig, B.; Landahl, E. C.; Peterson, E. R.; Rudati, J.; Santra, R.; Walko, D. A.; Young, L.

    2007-01-01

    Tunable, polarized, microfocused x-ray pulses were used to record x-ray absorption spectra across the K edges of Kr + and Kr 2+ produced by laser ionization of Kr. Prominent 1s→4p and 5p excitations are observed below the 1s ionization thresholds in accord with calculated transition energies and probabilities. Due to alignment of 4p hole states in the laser-ionization process, the Kr + 1s→4p cross section varies with respect to the angle between the laser and x-ray polarization vectors. This effect is used to determine the Kr + 4p 3/2 and 4p 1/2 quantum state populations, and these are compared with results of an adiabatic strong-field ionization theory that includes spin-orbit coupling

  14. Wavelengths of the Ni-like 4d to 4p X-ray laser lines

    International Nuclear Information System (INIS)

    Utsumi, Takayuki; Sasaki, Akira

    2000-01-01

    The wavelengths of the Ni-like 4d to 4p X-ray laser lines for elements ranging from Pd(Z=46) to U(Z=92) calculated using the relativistic multi-configuration Dirac-Fock code, i.e. grasp92, are presented. These optimal level calculations agree well with measurements and previous calculations. To obtain accurate lasing wavelengths is important to grasp the energy level structure of the complicated Ni-like ions, and especially for the development of collisionally pumped X-ray lasers. The lasing wavelengths are also essential to identify the lines and when the X-ray laser is utilized for imaging and interferometry. (author)

  15. X-ray flux and X-ray burn through experiments on reduced-scale targets at the Nif and OMEGA lasers

    International Nuclear Information System (INIS)

    Schneider, M.B.; Hinkel, D.E.; Young, B.K.; Holder, J.P.; Langdon, A.B.; Bower, D.E.; Bruns, H.C.; Campbell, K.M.; Celeste, J.R.; Compton, S.; Costa, R.L.; Dewald, E.L.; Dixit, S.N.; Eckart, M.J.; Eder, D.C.; Edwards, M.J.; Ellis, A.D.; Emig, J.A.; Froula, D.H.; Glebov, V.; Glenzer, S.H.; Hargrove, D.; Haynam, C.A.; Heeter, R.F.; Henesian, M.A.; Holtmeier, G.; James, D.L.; Jancaitis, K.S.; Kalantar, D.H.; Kamperschroer, J.H.; Kauffman, R.L.; Kimbrough, J.; Kirkwood, R.; Koniges, A.E.; Landen, O.L.; Landon, M.; Lee, F.D.; MacGowan, B.J.; Mackinnon, A.J.; Manes, K.R.; Marshall, C.; May, M.J.; McDonald, J.W.; Menapace, J.; Moon, S.J.; Moses, E.I.; Munro, D.H.; Murray, J.R.; Niemann, C.; Piston, K.; Power, G.D.; Rekow, V.; Ruppe, J.A.; Schein, J.; Shepherd, R.; Singh, M.S.; Sorce, C.; Springer, P.T.; Still, C.H.; Suter, L.J.; Tietbohl, G.L.; Turner, R.E.; Van Wonterghem, B.M.; Wallace, R.J.; Warrick, A.; Weber, F.; Wegner, P.J.; Williams, E.A.; Young, P.E.; Baldis, H.A.; Constantin, C.G.; Bahr, R.; Roberts, S.; Seka, W.; Stoeckl, C.; Pellinen, D.; Watts, P.

    2006-01-01

    An experimental campaign to maximize radiation drive in small-scale hohlraums has been carried out at the National Ignition Facility (NIF) at the Lawrence Livermore National Laboratory (Livermore, USA) and at the OMEGA laser at the Laboratory for Laser Energetics (Rochester, USA). The small-scale hohlraums, laser energy, laser pulse, and diagnostics were similar at both facilities but the geometries were very different. The NIF experiments used on-axis laser beams whereas the OMEGA experiments used 19 beams in three beam cones. In the cases when the lasers coupled well and produced similar radiation drive, images of X-ray burn-through and laser deposition indicate the pattern of plasma filling is very different. The OMEGA targets fill faster than the NIF targets, which helps explain the time behavior of the X-ray fluences. (authors)

  16. X-ray flux and X-ray burn through experiments on reduced-scale targets at the Nif and OMEGA lasers

    Energy Technology Data Exchange (ETDEWEB)

    Schneider, M.B.; Hinkel, D.E.; Young, B.K.; Holder, J.P.; Langdon, A.B.; Bower, D.E.; Bruns, H.C.; Campbell, K.M.; Celeste, J.R.; Compton, S.; Costa, R.L.; Dewald, E.L.; Dixit, S.N.; Eckart, M.J.; Eder, D.C.; Edwards, M.J.; Ellis, A.D.; Emig, J.A.; Froula, D.H.; Glebov, V.; Glenzer, S.H.; Hargrove, D.; Haynam, C.A.; Heeter, R.F.; Henesian, M.A.; Holtmeier, G.; James, D.L.; Jancaitis, K.S.; Kalantar, D.H.; Kamperschroer, J.H.; Kauffman, R.L.; Kimbrough, J.; Kirkwood, R.; Koniges, A.E.; Landen, O.L.; Landon, M.; Lee, F.D.; MacGowan, B.J.; Mackinnon, A.J.; Manes, K.R.; Marshall, C.; May, M.J.; McDonald, J.W.; Menapace, J.; Moon, S.J.; Moses, E.I.; Munro, D.H.; Murray, J.R.; Niemann, C.; Piston, K.; Power, G.D.; Rekow, V.; Ruppe, J.A.; Schein, J.; Shepherd, R.; Singh, M.S.; Sorce, C.; Springer, P.T.; Still, C.H.; Suter, L.J.; Tietbohl, G.L.; Turner, R.E.; Van Wonterghem, B.M.; Wallace, R.J.; Warrick, A.; Weber, F.; Wegner, P.J.; Williams, E.A.; Young, P.E. [Lawrence Livermore National Lab., Livermore, CA (United States); Baldis, H.A.; Constantin, C.G. [California at Davis Univ., CA (United States); Bahr, R.; Roberts, S.; Seka, W.; Stoeckl, C. [Laboratory for Laser Energetics, Rochester, NY (United States); Pellinen, D.; Watts, P. [Bechtel Nevada Corporation, Livermore, CA (United States)

    2006-06-15

    An experimental campaign to maximize radiation drive in small-scale hohlraums has been carried out at the National Ignition Facility (NIF) at the Lawrence Livermore National Laboratory (Livermore, USA) and at the OMEGA laser at the Laboratory for Laser Energetics (Rochester, USA). The small-scale hohlraums, laser energy, laser pulse, and diagnostics were similar at both facilities but the geometries were very different. The NIF experiments used on-axis laser beams whereas the OMEGA experiments used 19 beams in three beam cones. In the cases when the lasers coupled well and produced similar radiation drive, images of X-ray burn-through and laser deposition indicate the pattern of plasma filling is very different. The OMEGA targets fill faster than the NIF targets, which helps explain the time behavior of the X-ray fluences. (authors)

  17. Multimillijoule, highly coherent x-ray laser at 21 nm operating in deep saturation through double-pass amplification

    Czech Academy of Sciences Publication Activity Database

    Rus, Bedřich; Mocek, Tomáš; Präg R., Ansgar; Kozlová, Michaela; Jamelot, G.; Carillon, A.; Ros, D.; Joyeux, D.; Phalippou, D.

    2002-01-01

    Roč. 66, č. 6 (2002), s. 063806-1 - 063806-11 ISSN 1050-2947 R&D Projects: GA MŠk LN00A100; GA AV ČR IAA1010014 Institutional research plan: CEZ:AV0Z1010921 Keywords : x-ray lasers * laser plasma * x-ray spectroscopy x-ray optics Subject RIV: BH - Optics, Masers, Lasers Impact factor: 2.986, year: 2002

  18. Multi-millijoule, deeply saturated x-ray laser at 21.2 nm for applications in plasma physics

    Czech Academy of Sciences Publication Activity Database

    Rus, Bedřich; Mocek, Tomáš; Präg R., Ansgar; Kozlová, Michaela; Hudeček, Miroslav; Jamelot, G.; Carillon, A.; Ros, D.; Lagron, J.C.; Joyeux, D.; Phalippou, D.

    2002-01-01

    Roč. 44, - (2002), s. B207-B223 ISSN 0741-3335 R&D Projects: GA MŠk LN00A100; GA AV ČR IAA1010014 Institutional research plan: CEZ:AV0Z1010921 Keywords : x-ray lasers * laser plasma * x-ray spectroscopy * x-ray optics Subject RIV: BH - Optics, Masers, Lasers Impact factor: 2.121, year: 2002

  19. X-ray spectroscopy of plasmas created by the Nike KrF laser

    International Nuclear Information System (INIS)

    Aglitskiy, Y.; Lehecka, T.; Deniz, A.; Hardgrove, J.; Seely, J.; Brown, C.; Feldman, U.; Pawley, C.; Gerber, K.; Bodner, S.; Obenschain, S.; Lehmberg, R.; McLean, E.; Pronko, M.; Sethian, J.; Stamper, J.; Schmitt, A.; Sullivan, C.; Holland, G.; Laming, M.

    1997-01-01

    The x-ray emission from plasmas created by the Naval Research Laboratory Nike KrF laser was characterized using spectroscopic instruments. The targets were thin foils of aluminum and titanium and were irradiated by laser energies in the range 100 endash 1500 J. Using a spherical-crystal imaging spectrometer operating in the 1 endash 2 keV x-ray region, the density, temperature, and opacity of aluminum plasmas were determined with a spatial resolution of 10 μm in the direction perpendicular to the target surface. The spectral line ratios indicated that the aluminum plasmas were relatively dense, cool, and optically thick near the target surface

  20. Exploration of the fragmentation of laser shock-melted aluminum using x-ray backlighting

    Directory of Open Access Journals (Sweden)

    Lin Zhang

    2016-05-01

    Full Text Available The fragmentation of shock-melted metal material is an important scientific problem in shock physics and is suitable for experimentally investigating by the laser-driven x-ray backlighting technique. This letter reports on the exploration of laser shock-melted aluminum fragmentation by means of x-ray backlighting at the SGII high energy facility in China. High-quality and high-resolution radiographs with negligible motion blur were obtained and these images enabled analysis of the mass distribution of the fragmentation product.

  1. Modal study of refractive effects on x-ray laser coherence

    International Nuclear Information System (INIS)

    Amendt, P.; London, R.A.; Strauss, M.

    1991-01-01

    The role of smoothly varying transverse gain and refraction profiles on x-ray laser intensity and coherence is analyzed by modally expanding the electric field within the paraxial approximation. Comparison with a square transverse profile reveals that smooth-edged profiles lead to: (1) a greatly reduced number of guided modes, (2) the continued cancellation of local intensity from a loosely guided mode by resonant free modes, (3) and the absence of extraneous (or anomalous) free mode resonances. These generic spectral properties should enable a considerable simplification in analyzing and optimizing the coherence properties of laboratory soft x-ray lasers. 6 refs., 3 figs

  2. Analysis and implementation of a space resolving spherical crystal spectrometer for x-ray Thomson scattering experiments.

    Science.gov (United States)

    Harding, E C; Ao, T; Bailey, J E; Loisel, G; Sinars, D B; Geissel, M; Rochau, G A; Smith, I C

    2015-04-01

    The application of a space-resolving spectrometer to X-ray Thomson Scattering (XRTS) experiments has the potential to advance the study of warm dense matter. This has motivated the design of a spherical crystal spectrometer, which is a doubly focusing geometry with an overall high sensitivity and the capability of providing high-resolution, space-resolved spectra. A detailed analysis of the image fluence and crystal throughput in this geometry is carried out and analytical estimates of these quantities are presented. This analysis informed the design of a new spectrometer intended for future XRTS experiments on the Z-machine. The new spectrometer collects 6 keV x-rays with a spherically bent Ge (422) crystal and focuses the collected x-rays onto the Rowland circle. The spectrometer was built and then tested with a foam target. The resulting high-quality spectra prove that a spherical spectrometer is a viable diagnostic for XRTS experiments.

  3. A pin diode x-ray camera for laser fusion diagnostic imaging: Final technical report

    International Nuclear Information System (INIS)

    Jernigan, J.G.

    1987-01-01

    An x-ray camera has been constructed and tested for diagnostic imaging of laser fusion targets at the Laboratory for Laser Energetics (LLE) of the University of Rochester. The imaging detector, developed by the Hughes Aircraft Company, is a germanium PIN diode array of 10 x 64 separate elements which are bump bonded to a silicon readout chip containing a separate low noise amplifier for each pixel element. The camera assembly consists of a pinhole alignment mechanism, liquid nitrogen cryostat with detector mount and a thin beryllium entrance window, and a shielded rack containing the analog and digital electronics for operations. This x-ray camera has been tested on the OMEGA laser target chamber, the primary laser target facility of LLE, and operated via an Ethernet link to a SUN Microsystems workstation. X-ray images of laser targets are presented. The successful operation of this particular x-ray camera is a demonstration of the viability of the hybrid detector technology for future imaging and spectroscopic applications. This work was funded by the Department of Energy (DOE) as a project of the National Laser Users Facility (NLUF)

  4. X-ray polarization measurements at relativistic laser intensities

    International Nuclear Information System (INIS)

    Beiersdorfer, P.; Shepherd, R.; Mancini, R.C.

    2004-01-01

    An effort has been started to measure the short pulse laser absorption and energy partition at relativistic laser intensities up to 10 21 W/cm 2 . Plasma polarization spectroscopy is expected to play an important role in determining fast electron generation and measuring the electron distribution function. (author)

  5. Target surface structure effects on x-ray generation from laser produced plasma

    Energy Technology Data Exchange (ETDEWEB)

    Nishikawa, Tadashi; Nakano, Hidetoshi; Uesugi, Naoshi [NTT Basic Research Laboratories, Atsugi, Kanagawa (Japan)

    2000-03-01

    We demonstrated two different methods to increase the x-ray conversion efficiency of laser-produced plasma by modifying the target surface structure. One way is making a rectangular groove on a target surface and confining a laser-produced plasma in it. By the plasma collision process, a time and wavelength (4-10 nm) integrated soft x-ray fluence enhancement of 35 times was obtained at a groove width of 20 {mu}m and a groove depth of 100 {mu}m on a Nd-doped glass target. The other way is making an array of nanoholes on an alumina target and increasing the laser interaction depth with it. The x-ray fluence enhancement increases as the ionization level of Al becomes higher and the x-ray wavelength becomes shorter. Over 50-fold enhancement was obtained at a soft x-ray wavelength around 6 nm, which corresponds to the emission from Al{sup 8+,9+} ions. (author)

  6. Target surface structure effects on x-ray generation from laser produced plasma

    International Nuclear Information System (INIS)

    Nishikawa, Tadashi; Nakano, Hidetoshi; Uesugi, Naoshi

    2000-01-01

    We demonstrated two different methods to increase the x-ray conversion efficiency of laser-produced plasma by modifying the target surface structure. One way is making a rectangular groove on a target surface and confining a laser-produced plasma in it. By the plasma collision process, a time and wavelength (4-10 nm) integrated soft x-ray fluence enhancement of 35 times was obtained at a groove width of 20 μm and a groove depth of 100 μm on a Nd-doped glass target. The other way is making an array of nanoholes on an alumina target and increasing the laser interaction depth with it. The x-ray fluence enhancement increases as the ionization level of Al becomes higher and the x-ray wavelength becomes shorter. Over 50-fold enhancement was obtained at a soft x-ray wavelength around 6 nm, which corresponds to the emission from Al 8+,9+ ions. (author)

  7. From Storage Rings to Free Electron Lasers for Hard X-Rays

    International Nuclear Information System (INIS)

    Nuhn, H

    2004-01-01

    The intensity of X-ray sources has increased at a rapid rate since the late 1960s by 10 orders of magnitude and more through the use of synchrotron radiation produced by bending magnets, wigglers and undulators. Three generations of radiation sources have been identified depending on amplitude and quality of the radiation provided. While user facilities of the third generation were being constructed a new concept of radiation generating devices was being developed that offers an even larger increase in peak and average brightness than had been achieved till then. The new concept of the X-ray Free Electron Laser based on the principle of Self-Amplified Spontaneous Emission will be the basis of fourth generation X-ray source user facilities of this century. The paper will start with a brief history of the development of x-ray sources, discuss some of the differences between storage ring and free electron laser based approaches, and close with an update of the present development of x-ray free electron laser user facilities

  8. From Storage Rings to Free Electron Lasers for Hard X-Rays

    Energy Technology Data Exchange (ETDEWEB)

    Nuhn, H

    2004-01-09

    The intensity of X-ray sources has increased at a rapid rate since the late 1960s by 10 orders of magnitude and more through the use of synchrotron radiation produced by bending magnets, wigglers and undulators. Three generations of radiation sources have been identified depending on amplitude and quality of the radiation provided. While user facilities of the third generation were being constructed a new concept of radiation generating devices was being developed that offers an even larger increase in peak and average brightness than had been achieved till then. The new concept of the X-ray Free Electron Laser based on the principle of Self-Amplified Spontaneous Emission will be the basis of fourth generation X-ray source user facilities of this century. The paper will start with a brief history of the development of x-ray sources, discuss some of the differences between storage ring and free electron laser based approaches, and close with an update of the present development of x-ray free electron laser user facilities.

  9. A free-electron laser fourth-generation X-ray source

    International Nuclear Information System (INIS)

    Moncton, D. E.

    1999-01-01

    The field of synchrotrons radiation research has grown rapidly over the last 25 years due to both the push of the accelerator and magnet technology that produces the x-ray beams and the pull of the extraordinary scientific research those beams make possible. Three successive generations of synchrotrons radiation facilities have resulted in beam brilliances 11 to 12 orders of magnitude greater than the standard laboratory x-ray tube. However, greater advances can be easily imagined given the fact that x-ray beams from present-day facilities do not exhibit the coherence or time structure so familiar with the.optical laser. Theoretical work over the last ten years or so has pointed to the possibility of generating hard x-ray beams with laser-like characteristics. The concept is based on self-amplified spontaneous emission in free electron lasers. The use of a superconducting linac could produce a major, cost-effective facility that spans wavelengths from the ultraviolet to the hard x-ray regime, simultaneously servicing large numbers experimenters from a wide range of disciplines. As with each past generation of synchrotron facilities, immense new scientific opportunities from fourth-generation sources

  10. From storage rings to free electron lasers for hard x-rays

    International Nuclear Information System (INIS)

    Nuhn, Heinz-Dieter

    2004-01-01

    The intensity of x-ray sources has increased at a rapid rate since the late 1960s by ten orders of magnitude and more through the use of synchrotron radiation produced by bending magnets, wigglers and undulators. Three generations of radiation sources have been identified depending on amplitude and quality of the radiation provided. While user facilities of the third generation were being constructed, a new concept of radiation generating devices was being developed that offers an even larger increase in peak and average brightness than had been achieved till then. The new concept of the x-ray free electron laser based on the principle of self-amplified spontaneous emission will be the basis of fourth generation x-ray source user facilities of this century. The paper will start with a brief history of the development of x-ray sources, it will then discuss some of the differences between storage ring and free electron laser based approaches, and will close with an update of the present development of x-ray free electron laser user facilities

  11. Study of electrons distribution produced by laser-plasma interaction on x-ray generation

    International Nuclear Information System (INIS)

    Nikzad, L.; Sadighi-Bonabi, R.

    2010-01-01

    Complete text of publication follows. In the present work, X-ray beams are generated from interaction of relativistic electron beams produced by interaction of 500 mJ, 30 femtosecond Ti:sapphire laser pulses with thin solid targets such as lead, molybdenum and tungsten. After interaction of an intense pulsed laser with He gas-jet, a micron-scale laser produced plasma, creates and accelerates electron bunches, which propagate in the ion channel produced in the wake of the laser pulse. When an electron bunch is injected into the bubble in phase with its field, it will gain relativistic energies within very short distance. These accelerated electrons with Megaelectron-Volt energy and different distributions, can interact with targets to generate X-ray radiation with Kiloelectron-Volt energy, providing to be close enough to the gas-jet, where the relativistic accelerated electrons exist. Here, to determine the results, Monte Carlo simulation (MCNP-4C code) is employed to present Bremsstrahlung and characteristic X-ray production by quasi-Maxwellian and quasi-monoenergetic electron beams for three samples with different thicknesses. The outcome shows that for one specific electron spectrum and one definite target, the energy which the maximum characteristic x-ray flux takes place, varies with thickness. Also, for each material the energy which this maximum happens is constant for all thicknesses, for both produced electron spectra. For each sample, x-ray flux is calculated for different thicknesses and the thickness which the maximum characteristic x-ray flux occurs is obtained. Besides, it is concluded that by increasing the atomic number of the target, maximum X-ray flux moves towards higher energy. Also, comparison of the results for three targets and two electron distributions shows that by using quasi-monoenergetic electron spectra, more intense and narrower characteristic X-ray can be produced compared to the quasi-Maxwellian electron distribution, almost for all

  12. Diagnosing high density, fast-evolving plasmas using x-ray lasers

    International Nuclear Information System (INIS)

    Cauble, R.; Da Silva, L.B.; Barbee, T.W. Jr.

    1994-09-01

    As x-ray laser (XRL) research has matured, it has become possible to reliably utilize XRLs for applications in the laboratory. Laser coherence, high brightness and short pulse duration all make the XRL a unique tool for the diagnosis of laboratory plasmas. The high brightness of XRLs makes them well-suited for imaging and for interferometry when used in conjunction with multilayer mirrors and beamsplitters. We have utilized a soft x-ray laser in such an imaging system to examine laser-produced plasmas using radiography, moire deflectometry, and interferometry. Radiography experiments yield 100-200 ps snapshots of laser driven foils at a resolution of 1-2 μm. Moire deflectometry with an XRL has been used to probe plasmas at higher density than by optical means. Interferograms, which allow direct measurement of electron density in laser plasmas, have been obtained with this system

  13. Nearly copropagating sheared laser pulse FEL undulator for soft x-rays

    International Nuclear Information System (INIS)

    Lawler, J E; Yavuz, D; Bisognano, J; Bosch, R A; Chiang, T C; Green, M A; Jacobs, K; Miller, T; Wehlitz, R; York, R C

    2013-01-01

    A conceptual design for a soft x-ray free-electron laser (FEL) using a short-pulsed, high energy near infrared laser undulator and a low-emittance modest-energy (∼170 MeV) electron beam is described. This low-cost design uses the laser undulator beam in a nearly copropagating fashion with respect to the electron beam, instead of the traditional ‘head-on’ fashion. The nearly copropagating geometry reduces the Doppler shift of scattered radiation to yield soft, rather than hard x-rays. To increase the FEL gain a sheared laser pulse from a Ti : sapphire or other broadband laser is used to extend the otherwise short interaction time of the nearly copropagating laser undulator beam with a relativistic electron beam. (paper)

  14. Plasma polarization spectroscopy. Time resolved spectroscopy in soft x-ray region on recombining plasma

    International Nuclear Information System (INIS)

    Iwamae, Atsushi; Hasuo, Masahiro; Atake, Makoto; Hasegawa, Noboru; Kawachi, Tetsuya

    2007-01-01

    We present an experimental study of polarization of emission radiations from recombining plasmas generated by the interaction of 60 fs ultra-short laser pulses with a gas jet. Time-resolved spectroscopy with a temporal resolution of 5 ps with repetitive accumulation is used to follow the recombination time histories. (author)

  15. Measurement and analysis of thermal conductivity of isotopically controlled silicon layers by time-resolved X-ray scattering

    Energy Technology Data Exchange (ETDEWEB)

    Eon, S.; Frieling, R.; Bracht, H. [Institute for Materials Physics, University of Muenster, 48149 Muenster (Germany); Plech, A. [Institute for Photon Science and Synchrotron Radiation (IPS), 76344 Eggenstein-Leopoldshafen (Germany)

    2016-11-15

    Nanostructuring is considered to be an efficient way to tailor phonon scattering and to reduce the thermal conductivity while keeping good electronic properties. This can be ideally realized by mass modulation of chemical identical elements. In this work, we report measurements of the crossplane thermal conductivity of isotopically modulated {sup 28}Si/{sup 30}Si multilayer structures and of isotopically pure {sup 28}Si layers by means of time-resolved X-ray scattering. Compared to earlier investigations, an improved measurement technique has been applied to determine the cooling behavior of a top gold metal layer after laser excitation with picosecond time resolution until thermal equilibration is established. Detailed analysis of the cooling behavior not only confirms a reduced thermal conductivity of {sup 28}Si/{sup 30}Si multilayer structures compared to natural and isotopically enriched {sup 28}Si layers but also provides evidence of direct laser heating of the Si layer. This and extrinsic effects affecting the cooling behavior of the gold layer are taken into account to determine the thermal conductivity by means of the pump-and-probe measurement technique. (copyright 2016 WILEY-VCH Verlag GmbH and Co. KGaA, Weinheim)

  16. Homogenious focusing with a transient soft X-ray laser for irradiation experiments

    Czech Academy of Sciences Publication Activity Database

    Kazamias, S.; Cassou, K.; Guilbaud, O.; Klisnick, A.; Ros, D.; Plé, F.; Jamelot, G.; Rus, Bedřich; Kozlová, Michaela; Stupka, Michal; Mocek, Tomáš; Douillet, D.; Zeitoun, P.; Joyeux, D.; Phalippou, D.

    2006-01-01

    Roč. 263, - (2006), s. 98-104 ISSN 0030-4018 R&D Projects: GA MŠk(CZ) LC528; GA ČR GA202/05/2316 Institutional research plan: CEZ:AV0Z10100523 Keywords : soft X-Ray laser * focusing * laser plasma * UV radiation * beam profile Subject RIV: BH - Optics, Masers, Lasers Impact factor: 1.480, year: 2006

  17. Single-particle coherent diffractive imaging with a soft x-ray free electron laser: towards soot aerosol morphology

    International Nuclear Information System (INIS)

    Bogan, Michael J; Starodub, Dmitri; Hampton, Christina Y; Sierra, Raymond G

    2010-01-01

    The first of its kind, the Free electron LASer facility in Hamburg, FLASH, produces soft x-ray pulses with unprecedented properties (10 fs, 6.8-47 nm, 10 12 photons per pulse, 20 μm diameter). One of the seminal FLASH experiments is single-pulse coherent x-ray diffractive imaging (CXDI). CXDI utilizes the ultrafast and ultrabright pulses to overcome resolution limitations in x-ray microscopy imposed by x-ray-induced damage to the sample by 'diffracting before destroying' the sample on sub-picosecond timescales. For many lensless imaging algorithms used for CXDI it is convenient when the data satisfy an oversampling constraint that requires the sample to be an isolated object, i.e. an individual 'free-standing' portion of disordered matter delivered to the centre of the x-ray focus. By definition, this type of matter is an aerosol. This paper will describe the role of aerosol science methodologies used for the validation of the 'diffract before destroy' hypothesis and the execution of the first single-particle CXDI experiments being developed for biological imaging. FLASH CXDI now enables the highest resolution imaging of single micron-sized or smaller airborne particulate matter to date while preserving the native substrate-free state of the aerosol. Electron microscopy offers higher resolution for single-particle analysis but the aerosol must be captured on a substrate, potentially modifying the particle morphology. Thus, FLASH is poised to contribute significant advancements in our knowledge of aerosol morphology and dynamics. As an example, we simulate CXDI of combustion particle (soot) morphology and introduce the concept of extracting radius of gyration of fractal aggregates from single-pulse x-ray diffraction data. Future upgrades to FLASH will enable higher spatially and temporally resolved single-particle aerosol dynamics studies, filling a critical technological need in aerosol science and nanotechnology. Many of the methodologies described for FLASH will

  18. Grain-resolved elastic strains in deformed copper measured by three-dimensional X-ray diffraction

    DEFF Research Database (Denmark)

    Oddershede, Jette; Schmidt, Søren; Poulsen, Henning Friis

    2011-01-01

    This X-ray diffraction study reports the grain-resolved elastic strains in about 1000 randomly oriented grains embedded in a polycrystalline copper sample. Diffraction data were collected in situ in the undeformed state and at a plastic strain of 1.5% while the sample was under tensile load...

  19. Laser-Hole Boring into Overdense Plasmas Measured with Soft X-Ray Laser Probing

    Energy Technology Data Exchange (ETDEWEB)

    Takahashi, K [Institute of Laser Engineering, Osaka University, Yamada Oka 2-6, Suita, Osaka 565-0871, (Japan); Kodama, R [Institute of Laser Engineering, Osaka University, Yamada Oka 2-6, Suita, Osaka 565-0871, (Japan); Tanaka, K A [Institute of Laser Engineering, Osaka University, Yamada Oka 2-6, Suita, Osaka 565-0871, (Japan); Hashimoto, H [Institute of Laser Engineering, Osaka University, Yamada Oka 2-6, Suita, Osaka 565-0871, (Japan); Kato, Y [Institute of Laser Engineering, Osaka University, Yamada Oka 2-6, Suita, Osaka 565-0871, (Japan); Mima, K [Institute of Laser Engineering, Osaka University, Yamada Oka 2-6, Suita, Osaka 565-0871, (Japan); Weber, F A [University of California, Lawrence Livermore National Laboratory, P.O. Box 808, Livermore, California 94550 (United States); Barbee, Jr, T W [University of California, Lawrence Livermore National Laboratory, P.O. Box 808, Livermore, California 94550 (United States); Da Silva, L B [University of California, Lawrence Livermore National Laboratory, P.O. Box 808, Livermore, California 94550 (United States)

    2000-03-13

    A laser self-focused channel formation into overdense plasmas was observed using a soft x-ray laser probe system with a grid image refractometry (GIR) technique. 1.053 {mu}m laser light with a 100 ps pulse duration was focused onto a preformed plasma at an intensity of 2x10{sup 17} W /cm{sup 2} . Cross sections of the channel were obtained which show a 30 {mu}m diameter in overdense plasmas. The channel width in the overdense region was kept narrow as a result of self-focusing. Conically diverging density ridges were also observed along the channel, indicating a Mach cone created by a shock wave due to the supersonic propagation of the channel front. (c) 2000 The American Physical Society.

  20. Laser-Hole Boring into Overdense Plasmas Measured with Soft X-Ray Laser Probing

    International Nuclear Information System (INIS)

    Takahashi, K.; Kodama, R.; Tanaka, K. A.; Hashimoto, H.; Kato, Y.; Mima, K.; Weber, F. A.; Barbee, T. W. Jr.; Da Silva, L. B.

    2000-01-01

    A laser self-focused channel formation into overdense plasmas was observed using a soft x-ray laser probe system with a grid image refractometry (GIR) technique. 1.053 μm laser light with a 100 ps pulse duration was focused onto a preformed plasma at an intensity of 2x10 17 W /cm 2 . Cross sections of the channel were obtained which show a 30 μm diameter in overdense plasmas. The channel width in the overdense region was kept narrow as a result of self-focusing. Conically diverging density ridges were also observed along the channel, indicating a Mach cone created by a shock wave due to the supersonic propagation of the channel front. (c) 2000 The American Physical Society

  1. Synchrotron radiation and free-electron lasers principles of coherent X-ray generation

    CERN Document Server

    Kim, Kwang-Je; Lindberg, Ryan

    2017-01-01

    Learn about the latest advances in high-brightness X-ray physics and technology with this authoritative text. Drawing upon the most recent theoretical developments, pre-eminent leaders in the field guide readers through the fundamental principles and techniques of high-brightness X-ray generation from both synchrotron and free-electron laser sources. A wide range of topics is covered, including high-brightness synchrotron radiation from undulators, self-amplified spontaneous emission, seeded high-gain amplifiers with harmonic generation, ultra-short pulses, tapering for higher power, free-electron laser oscillators, and X-ray oscillator and amplifier configuration. Novel mathematical approaches and numerous figures accompanied by intuitive explanations enable easy understanding of key concepts, whilst practical considerations of performance-improving techniques and discussion of recent experimental results provide the tools and knowledge needed to address current research problems in the field. This is a comp...

  2. Ultrafast laser pump X-ray probe experiments by means of asynchronous sampling

    International Nuclear Information System (INIS)

    Issenmann, D; Ibrahimkutty, S; Baumbach, T; Müller, A-S; Plech, A; Steininger, R; Göttlicher, J; Hiller, N

    2013-01-01

    A high time resolution in the picosecond range is required for the time-domain investigation of phonon dynamics in crystalline systems. Following a recently developed scheme in the visible spectrum, this resolution can be achieved by a method called asynchronous optical x-ray sampling (ASOXS). A pulsed femtosecond laser with high repetition rate is synchronized to the electron bunches in a storage ring. A slight frequency detuning changes the mutual delay continuously, resulting in a time-domain x-ray sampling of the laser-excited system. At the synchrotron radiation source ANKA a machine mode with low momentum compaction factor α c is available, which delivers ultra-short x-ray pulses in the picosecond range.

  3. Overview of the ARGOS X-ray framing camera for Laser MegaJoule

    Energy Technology Data Exchange (ETDEWEB)

    Trosseille, C., E-mail: clement.trosseille@cea.fr; Aubert, D.; Auger, L.; Bazzoli, S.; Brunel, P.; Burillo, M.; Chollet, C.; Jasmin, S.; Maruenda, P.; Moreau, I.; Oudot, G.; Raimbourg, J.; Soullié, G.; Stemmler, P.; Zuber, C. [CEA, DAM, DIF, F-91297 Arpajon (France); Beck, T. [CEA, DEN, CADARACHE, F-13108 St Paul lez Durance (France); Gazave, J. [CEA, DAM, CESTA, F-33116 Le Barp (France)

    2014-11-15

    Commissariat à l’Énergie Atomique et aux Énergies Alternatives has developed the ARGOS X-ray framing camera to perform two-dimensional, high-timing resolution imaging of an imploding target on the French high-power laser facility Laser MegaJoule. The main features of this camera are: a microchannel plate gated X-ray detector, a spring-loaded CCD camera that maintains proximity focus in any orientation, and electronics packages that provide remotely-selectable high-voltages to modify the exposure-time of the camera. These components are integrated into an “air-box” that protects them from the harsh environmental conditions. A miniaturized X-ray generator is also part of the device for in situ self-testing purposes.

  4. Obtaining attosecond x-ray pulses using a self-amplified spontaneous emission free electron laser

    Directory of Open Access Journals (Sweden)

    A. A. Zholents

    2005-05-01

    Full Text Available We describe a technique for the generation of a solitary attosecond x-ray pulse in a free-electron laser (FEL, via a process of self-amplified spontaneous emission. In this method, electrons experience an energy modulation upon interacting with laser pulses having a duration of a few cycles within single-period wiggler magnets. Two consecutive modulation sections, followed by compression in a dispersive section, are used to obtain a single, subfemtosecond spike in the electron peak current. This region of the electron beam experiences an enhanced growth rate for FEL amplification. After propagation through a long undulator, this current spike emits a ∼250   attosecond x-ray pulse whose intensity dominates the x-ray emission from the rest of the electron bunch.

  5. Feasibility analysis for attosecond X-ray pulses at FERMI@ELETTRA free electron laser

    Energy Technology Data Exchange (ETDEWEB)

    Zholents, Alexander

    2004-09-01

    We present preliminary analysis for the feasibility of the attosecond x-ray pulses at a proposed FERMI@ELETTRA free electron laser (FEL) [1]. In part 1 we restrict ourselves to minimal modifications to the proposed FEL and consider a scheme for attosecond x-ray production which can be qualified as a small add-on to a primary facility. We demonstrate that at 5-nm wavelength our scheme is capable for production of pulses with an approximate duration of 100 attoseconds at approximately 2 MW peak power and with an absolute temporal synchronization to a pump laser pulse. In part 2 we propose to use an FEL amplifier seeded by a VUV signal and to follow it by the scheme for attosecond x-ray production described in part 1.

  6. Pixel array detector for X-ray free electron laser experiments

    Energy Technology Data Exchange (ETDEWEB)

    Philipp, Hugh T., E-mail: htp2@cornell.edu [Department of Physics, Laboratory of Solid State Physics, Cornell University, Ithaca, NY 14853 (United States); Hromalik, Marianne [Electrical and Computer Engineering, SUNY Oswego, Oswego, NY 13126 (United States); Tate, Mark; Koerner, Lucas [Department of Physics, Laboratory of Solid State Physics, Cornell University, Ithaca, NY 14853 (United States); Gruner, Sol M. [Department of Physics, Laboratory of Solid State Physics, Cornell University, Ithaca, NY 14853 (United States); Wilson Laboratory, Cornell University, CHESS, Ithaca, NY 14853 (United States)

    2011-09-01

    X-ray free electron lasers (XFELs) promise to revolutionize X-ray science with extremely high peak brilliances and femtosecond X-ray pulses. This will require novel detectors to fully realize the potential of these new sources. There are many current detector development projects aimed at the many challenges of meeting the XFEL requirements . This paper describes a pixel array detector (PAD) that has been developed for the Coherent X-ray Imaging experiment at the Linac Coherent Light Source (LCLS) at the SLAC National Laboratory . The detector features 14-bit in-pixel digitization; a 2-level in-pixel gain setting that can be used to make an arbitrary 2-D gain pattern that is adaptable to a particular experiment; the ability to handle instantaneous X-ray flux rates of 10{sup 17} photons per second; and continuous frames rates in excess of 120 Hz. The detector uses direct detection of X-rays in a silicon diode. The charge produced by the diode is integrated in a pixilated application specific integrated circuit (ASIC) which digitizes collected holes with single X-ray photon capability. Each ASIC is 194x185 pixels, each pixel is 110{mu}mx110{mu}m on a side. Each pixel can detect up to 2500 X-rays per frame in low-gain mode, yet easily detects single photons at high-gain. Cooled, single-chip detectors have been built and meet all the required specifications. SLAC National Laboratory is engaged in constructing a tiled, multi-chip 1516x1516 pixel detector.

  7. Time-Resolved X-Ray Diffraction: The Dynamics of the Chemical Bond

    DEFF Research Database (Denmark)

    Møller, Klaus Braagaard; Henriksen, Niels Engholm

    2012-01-01

    We review the basic theoretical formulation for pulsed X-ray scattering on nonstationary molecular states. Relevant time scales are discussed for coherent as well as incpherent X-ray pulses. The general formalism is applied to a nonstationary diatomic molecule in order to highlight the relation b...

  8. Pore-scale evaporation-condensation dynamics resolved by synchrotron x-ray tomography.

    Science.gov (United States)

    Shahraeeni, Ebrahim; Or, Dani

    2012-01-01

    Capillary processes greatly influence vapor mediated transport dynamics and associated changes in liquid phase content of porous media. Rapid x-ray synchrotron tomography measurements were used to resolve liquid-vapor interfacial dynamics during evaporation and condensation within submillimetric pores forming between sintered glass bead samples subjected to controlled ambient temperature and relative humidity. Evolution of gas-liquid interfacial shapes were in agreement with predictions based on our analytical model for interfacial dynamics in confined wedge-shaped pores. We also compared literature experimental data at the nanoscale to illustrate the capability of our model to describe early stages of condensation giving rise to the onset of capillary forces between rough surfaces. The study provides high resolution, synchrotron-based observations of capillary evaporation-condensation dynamics at the pore scale as the confirmation of the pore scale analytical model for capillary condensation in a pore and enables direct links with evolution of macroscopic vapor gradients within a sintered glass bead sample through their effect on configuration and evolution of the local interfaces. Rapid condensation processes play a critical role in the onset of capillary-induced friction affecting mechanical behavior of physical systems and industrial applications.

  9. Development of Compact Soft X-ray Source Based on Laser Undulator

    CERN Document Server

    Kuroda, Ryunosuke; Minamiguchi, S; Saitô, T; Ueyama, D; Washio, Masakazu

    2004-01-01

    A compact soft X-ray source is required in various research fields such as material and biological science. The laser undulator based on backward Compton scattering has been developed as a compact soft X-ray source for the biological observation at Waseda University. It is performed in a water window region (250eV - 500 eV) using the interaction between 1047 nm Nd:YLF laser and 4 MeV high quality electron beam generated from rf gun system. The range of energy in the water window region has K-shell absorption edges of Oxygen, Carbon and Nitrogen, which mainly constitute of living body. Since the absorption coefficient of water is much smaller than the protein’s coefficient in this range, a dehydration of the specimens is not necessary. As a preliminary experiment, about 300 eV X-ray generation was carried out. As next step, soft X-ray optics with zone plate was proposed for Soft X-ray microscopy. In this conference, we will report details and results of the experiment.

  10. X-ray comb generation from nuclear-resonance-stabilized x-ray free-electron laser oscillator for fundamental physics and precision metrology

    Directory of Open Access Journals (Sweden)

    B. W. Adams

    2015-03-01

    Full Text Available An x-ray free-electron laser oscillator (XFELO is a next-generation x-ray source, similar to free-electron laser oscillators at VUV and longer wavelengths but using crystals as high-reflectivity x-ray mirrors. Each output pulse from an XFELO is fully coherent with high spectral purity. The temporal coherence length can further be increased drastically, from picoseconds to microseconds or even longer, by phase-locking successive XFELO output pulses, using the narrow nuclear resonance lines of nuclei such as ^{57}Fe as a reference. We show that the phase fluctuation due to the seismic activities is controllable and that due to spontaneous emission is small. The fluctuation of electron-bunch spacing contributes mainly to the envelope fluctuation but not to the phase fluctuation. By counting the number of standing-wave maxima formed by the output of the nuclear-resonance-stabilized (NRS XFELO over an optically known length, the wavelength of the nuclear resonance can be accurately measured, possibly leading to a new length or frequency standard at x-ray wavelengths. A NRS-XFELO will be an ideal source for experimental x-ray quantum optics as well as other fundamental physics. The technique can be refined for other, narrower resonances such as ^{181}Ta or ^{45}Sc.

  11. Compact gain saturated plasma based X-ray lasers down to 6.9nm

    Science.gov (United States)

    Rocca, Jorge; Wang, Y.; Wang, S.; Rockwood, A.; Berrill, M.; Shlyaptsev, V.

    2017-10-01

    Plasma based soft x-ray amplifiers allow many experiments requiring bright, high energy soft x-ray laser pulses to be conducted in compact facilities. We have extended the wavelength of compact gain saturated x-ray lasers to 6.89 nm in a Ni-like Gd plasma generated by a Ti:Sa laser. Gain saturated laser operation was also obtained at 7.36 nm in Ni-like Sm. Isolectronic scaling and optimization of laser pre-pulse duration allowed us to also observe strong lasing at 6.6 nm and 6.1 nm in Ni-like Tb, and amplification at 6.4 nm and 5.89 nm in Ni-like Dy. The results were obtained by transient laser heating of solid targets with traveling wave excitation at progressively increased gracing incidence angles. We show that the optimum pump angle of incidence for collisional Ni-like lasers increases linearly with atomic number from Z =42 to Z =66, reaching 43 degrees for Ni-like Dy, in good agreement with hydrodynamic/atomic physics simulations. These results will enable single-shot nano-scale imaging and other application of sub-7 nm lasers to be performed at compact facilities. Work supported by Grant DE-FG02-4ER15592 of the Department of Energy, Office of Science, and by the National Science Foundation Grant ECCS 1509925.

  12. Ultra fast x-ray streak camera

    International Nuclear Information System (INIS)

    Coleman, L.W.; McConaghy, C.F.

    1975-01-01

    A unique ultrafast x-ray sensitive streak camera, with a time resolution of 50psec, has been built and operated. A 100A thick gold photocathode on a beryllium vacuum window is used in a modified commerical image converter tube. The X-ray streak camera has been used in experiments to observe time resolved emission from laser-produced plasmas. (author)

  13. Micro-fresnel structures for microscopy of laser generated bright x-ray sources

    International Nuclear Information System (INIS)

    Ceglio, N.M.; Shavers, D.C.; Flanders, D.C.; Smith, H.I.

    1979-01-01

    A brief parametric survey of the x-ray characteristics of a gold micro-disk irradiated at 3 x 10 14 watt/cm 2 by a 1 nsec Nd-glass laser pulse has been provided as an example of a laser generated bright x-ray source. It was shown that a simple phenomenological model of the laser generated x-ray source as a microscopic equilibrium plasma radiating as a blackbody for a finite time determined by its hydrodynamic disassembly and radiation losses, serves to provide an adequate approximation to the x-ray characteristics of such sources. The current state of x-ray microscopy within the LLL laser fusion program was briefly reviewed. Kirpatrick--Baez grazing incidence reflection x-ray microscopes are being used to provide 3 to 5 μm resolution, broadband images (ΔE/E approx. 0.3) over a spectral range from .6 keV to 3.5 keV. Zone Plate Coded Imaging is used to provide 5 to 10 μm resolution, broadband (ΔE/E approx. 0.5) images over a spectral range from 3 keV to 50 keV. Efficient x-ray lensing elements with anticipated submicron resolution are being developed for narrowband (ΔE/E approx. 10 -2 ) imaging applications over a spectral range .1 keV to 8 keV. The x-ray lens design is that of a transmission blazed Fresnel phase plate. Micro--Fresnel zone plates with 3200 A minimum linewidth have been fabricated and preliminary resolution tests begun. The first resolution test pattern, having minimum linewidth of 2.5 μm, was imaged in lambda = 8.34 A light with no difficulty. Newer test patterns with submicron minimum line are being prepared for the next stage of resolution testing. An off-axis Fresnel zone plate with 1600 A minimum linewidth is presently being fabricated for use as an imaging spectrometer in order to provide spatially separated, chromatically distinct images of characteristic line emissions from laser fusion targets

  14. Controlled molecules for X-ray diffraction experiments at free-electron lasers

    International Nuclear Information System (INIS)

    Stern, Stephan

    2013-12-01

    X-ray diffractive imaging is at the very heart of materials science and has been utilized for decades to solve unknown molecular structures. Nowadays, it serves as the key method of structural biology to solve molecular structures of large biological molecules comprising several thousand or even millions of atoms. However, X-ray diffraction from isolated molecules is very weak. Therefore, the regular and periodic arrangement of a huge number of identical copies of a certain molecule of interest within a crystal lattice has been a necessary condition in order to exploit Bragg diffraction of X-rays. This results in a huge increase in scattered signal and a strongly improved signal-to-noise ratio compared to diffraction from non-crystalline samples. The major bottleneck of structural biology is that many of biologically interesting molecules refuse to form crystals of sufficient size to be used at synchrotron X-ray lightsources. However, novel X-ray free-electron lasers (XFELs), which became operational very recently, promise to address this issue. X-ray pulses provided by XFELs are many orders of magnitude more intense than X-ray pulses from a synchrotron source and at the same time as short as only several tens of femtoseconds. Combined with wavelengths in the nm-pm range, XFELs are well-suited to study ultrafast atomic and molecular dynamics. Additionally, the ultrashort pulses can be utilized to circumvent the damage threshold which set a limit to the incident intensity in X-ray diffraction experiments before. At XFELs, though eventually destroying the investigated sample, no significant sample deterioration happens on the ultrashort timescale of the XFEL pulse and the measured diffraction pattern is due to an (almost) unharmed sample. In the framework of this thesis, the approach of utilizing the highly intense XFEL pulses for X-ray diffraction of weakly-scattering non-crystalline samples was taken to the limit of small isolated molecules. X-ray diffraction was

  15. Controlled molecules for X-ray diffraction experiments at free-electron lasers

    Energy Technology Data Exchange (ETDEWEB)

    Stern, Stephan

    2013-12-15

    X-ray diffractive imaging is at the very heart of materials science and has been utilized for decades to solve unknown molecular structures. Nowadays, it serves as the key method of structural biology to solve molecular structures of large biological molecules comprising several thousand or even millions of atoms. However, X-ray diffraction from isolated molecules is very weak. Therefore, the regular and periodic arrangement of a huge number of identical copies of a certain molecule of interest within a crystal lattice has been a necessary condition in order to exploit Bragg diffraction of X-rays. This results in a huge increase in scattered signal and a strongly improved signal-to-noise ratio compared to diffraction from non-crystalline samples. The major bottleneck of structural biology is that many of biologically interesting molecules refuse to form crystals of sufficient size to be used at synchrotron X-ray lightsources. However, novel X-ray free-electron lasers (XFELs), which became operational very recently, promise to address this issue. X-ray pulses provided by XFELs are many orders of magnitude more intense than X-ray pulses from a synchrotron source and at the same time as short as only several tens of femtoseconds. Combined with wavelengths in the nm-pm range, XFELs are well-suited to study ultrafast atomic and molecular dynamics. Additionally, the ultrashort pulses can be utilized to circumvent the damage threshold which set a limit to the incident intensity in X-ray diffraction experiments before. At XFELs, though eventually destroying the investigated sample, no significant sample deterioration happens on the ultrashort timescale of the XFEL pulse and the measured diffraction pattern is due to an (almost) unharmed sample. In the framework of this thesis, the approach of utilizing the highly intense XFEL pulses for X-ray diffraction of weakly-scattering non-crystalline samples was taken to the limit of small isolated molecules. X-ray diffraction was

  16. Generation of plasma X-ray sources via high repetition rate femtosecond laser pulses

    Science.gov (United States)

    Baguckis, Artūras; Plukis, Artūras; Reklaitis, Jonas; Remeikis, Vidmantas; Giniūnas, Linas; Vengris, Mikas

    2017-12-01

    In this study, we present the development and characterization of Cu plasma X-ray source driven by 20 W average power high repetition rate femtosecond laser in ambient atmosphere environment. The peak Cu- Kα photon flux of 2.3 × 109 photons/s into full solid angle is demonstrated (with a process conversion efficiency of 10-7), using pulses with peak intensity of 4.65 × 1014 W/cm2. Such Cu- Kα flux is significantly larger than others found in comparable experiments, performed in air environment. The effects of resonance plasma absorption process, when optimized, are shown to increase measured flux by the factor of 2-3. The relationship between X-ray photon flux and plasma-driving pulse repetition rate is quasi-linear, suggesting that fluxes could further be increased to 1010 photons/s using even higher average powers of driving radiation. These results suggest that to fully utilize the potential of high repetition rate laser sources, novel target material delivery systems (for example, jet-based ones) are required. On the other hand, this study demonstrates that high energy lasers currently used for plasma X-ray sources can be conveniently and efficiently replaced by high average power and repetition rate laser radiation, as a way to increase the brightness of the generated X-rays.

  17. Optimization of soft x-ray line emission from laser-produced carbon ...

    Indian Academy of Sciences (India)

    Intense XUV soft x-ray emission from laser-produced plasma sources is currently ... absorption edges of oxygen and carbon respectively) is particularly attractive as it permits ... ability of the target element producing intense discrete lines in the water .... ficient due to Pert [17] and dielectronic recombination coefficient due to ...

  18. Absorption of aluminium X-ray lines in a laser created gold plasma

    International Nuclear Information System (INIS)

    Combis, P.; Busquet, M.; Louis-Jacquet, M.

    1986-04-01

    We have studied the absorption of aluminium X-ray lines through a gold plasma by focusing a high intensity laser-beam onto a specific target. Absorption in the wavelength range of 5 to 7 A has been evidenced and measured for Aluminium resonance lines

  19. Electron beam requirements for soft x-ray/XUV free-electron lasers

    International Nuclear Information System (INIS)

    Goldstein, J.C.

    1987-01-01

    A discussion of the electron beam quality (peak current, energy spread, and transverse emittance) required to drive short wavelength free-electron lasers in the XUV (10-100 nm) and soft x-ray (<10 nm) optical wavelength ranges is presented

  20. High pressure X-ray preionized TEMA-CO2 laser

    NARCIS (Netherlands)

    Bonnie, R.J.M.; Witteman, W.J.

    1987-01-01

    The construction of a high-pressure (up to 20 atm) transversely excited CO2 laser using transverse X-ray preionization is described. High pressure operation was found to be greatly improved in comparison to UV-preionized systems. Homogeneous discharges have been achieved in the pressure range 5–20

  1. Toward atomic resolution diffractive imaging of isolated molecules with x-ray free-electron lasers

    DEFF Research Database (Denmark)

    Stern, Stephan; Holmegaard, Lotte; Filsinger, Frank

    2014-01-01

    We give a detailed account of the theoretical analysis and the experimental results of an x-ray-diffraction experiment on quantum-state selected and strongly laser-aligned gas-phase ensembles of the prototypical large asymmetric rotor molecule 2,5-diiodobenzonitrile, performed at the Linac Cohere...

  2. Compact tunable Compton x-ray source from laser-plasma accelerator and plasma mirror

    International Nuclear Information System (INIS)

    Tsai, Hai-En; Wang, Xiaoming; Shaw, Joseph M.; Li, Zhengyan; Zgadzaj, Rafal; Henderson, Watson; Downer, M. C.; Arefiev, Alexey V.; Zhang, Xi; Khudik, V.; Shvets, G.

    2015-01-01

    We present an in-depth experimental-computational study of the parameters necessary to optimize a tunable, quasi-monoenergetic, efficient, low-background Compton backscattering (CBS) x-ray source that is based on the self-aligned combination of a laser-plasma accelerator (LPA) and a plasma mirror (PM). The main findings are (1) an LPA driven in the blowout regime by 30 TW, 30 fs laser pulses produce not only a high-quality, tunable, quasi-monoenergetic electron beam, but also a high-quality, relativistically intense (a 0 ∼ 1) spent drive pulse that remains stable in profile and intensity over the LPA tuning range. (2) A thin plastic film near the gas jet exit retro-reflects the spent drive pulse efficiently into oncoming electrons to produce CBS x-rays without detectable bremsstrahlung background. Meanwhile, anomalous far-field divergence of the retro-reflected light demonstrates relativistic “denting” of the PM. Exploiting these optimized LPA and PM conditions, we demonstrate quasi-monoenergetic (50% FWHM energy spread), tunable (75–200 KeV) CBS x-rays, characteristics previously achieved only on more powerful laser systems by CBS of a split-off, counter-propagating pulse. Moreover, laser-to-x-ray photon conversion efficiency (∼6 × 10 −12 ) exceeds that of any previous LPA-based quasi-monoenergetic Compton source. Particle-in-cell simulations agree well with the measurements

  3. Short-time X-ray diffraction with an efficient-optimized, high repetition-rate laser-plasma X-ray-source

    International Nuclear Information System (INIS)

    Kaehle, Stephan

    2009-01-01

    This thesis deals with the production and application of ultrashort X-ray pulses. In the beginning different possibilities for the production of X-ray pulses with pulse durations of below one picosecond are presented, whereby the main topic lies on the so called laser-plasma X-ray sources with high repetition rate. In this case ultrashort laser pulses are focused on a metal, so that in the focus intensities of above 10 16 W/cm 2 dominate. In the ideal case in such way ultrafast electrons are produced, which are responsible for line radiation. In these experiments titanium K α radiation is produced, thes photons possess an energy of 4.51 keV. For the efficient production of line radiation here the Ti:Sa laser is optimized in view of the laser energy and the pulse shape and the influence of the different parameters on the K α production systematically studied. The influences of laser intensity, system-conditioned pre-pulses and of phase modulation are checked. It turns out that beside the increasement of the K α radiation by a suited laser intensity a reduction of the X-ray background radiation is of deciding importance for the obtaining of clear diffraction images. This background radiation is mainly composed of bremsstrahlung. It can be suppressed by the avoidance of intrinsic pre-pulses and by means of 2nd-order phase modulation. By means of optical excitation and X-ray exploration experiments the production of acoustic waves after ultrashort optical excitation in a 150 nm thick Ge(111) film on Si(111) is studied. These acoustic waves are driven by thermal (in this time scale time-independent) and electronic (time dependent) pressure amounts. As essential results it turns out that the relative amount of the electronic pressure increases with decreasing excitation density [de

  4. Temporal and Spatial Shaping of X-Ray Free-Electron Lasers

    Energy Technology Data Exchange (ETDEWEB)

    Guo, G [SLAC National Accelerator Lab., Menlo Park, CA (United States); Marinelli, AGOSTINO

    2018-04-01

    The x-ray free-elec­tron laser is the bright­est source of x-rays, with a peak bright­ness ten or­ders of mag­ni­tude higher than con­ven­tional syn­chro­tron ra­di­a­tion sources. Much like con­ven­tional lasers, XFELs are ex­tremely flex­i­ble ma­chines and the prop­er­ties of the x-rays can be con­trolled by ac­cu­rately ma­nip­u­lat­ing the las­ing medium, i.e. the elec­tron beam. In my talk I will dis­cuss past and pre­sent re­search on shap­ing the tem­po­ral prop­er­ties of the x-rays at the Linac Co­her­ent Light Source (LCLS). I will dis­cuss the two-color FEL modes and their ap­pli­ca­tions in user ex­per­i­ments. Fi­nally I will pre­sent our re­sults on laser-shap­ing of x-ray pulses and our plans for at­tosec­ond op­er­a­tion in the soft x-ray regime.

  5. Selenium x-ray laser line profile measurements

    International Nuclear Information System (INIS)

    Koch, J.A.; MacGowan, B.J.; Da Silva, L.; Matthews, D.L.; Mrowka, S.; Underwood, J.H.; Batson, P.J.

    1992-01-01

    We discuss our recent measurements of the spectral width of the 206.38 Angstrom laser in Ne-like Se. These measurements were performed over a wide range of amplifier length indicate an intrinsic line width of 50 m Angstrom FWHM (full-width at half-maximum), show gain narrowing to 10 m Angstrom in intermediate length amplifiers and show no significant re-broadening in We briefly discuss the experiments and interpretations

  6. Development of a fast pixel array detector for use in microsecond time-resolved x-ray diffraction

    International Nuclear Information System (INIS)

    Barna, S.L.; Gruner, S.M.; Shepherd, J.A.

    1995-01-01

    A large-area pixel x-ray detector is being developed to collect eight successive frames of wide dynamic range two-dimensional images at 200kHz rates. Such a detector, in conjunction with a synchrotron radiation x-ray source, will enable time-resolved x-ray studies of proteins and other materials on time scales which have previously been inaccessible. The detector will consist of an array of fully-depleted 150 micron square diodes connected to a CMOS integrated electronics layer with solder bump-bonding. During each framing period, the current resulting from the x-rays stopped in the diodes is integrated in the electronics layer, and then stored in one of eight storage capacitors underneath the pixel. After the last frame, the capacitors are read out at standard data transmission rates. The detector has been designed for a well-depth of at least 10,000 x-rays (at 20keV), and a noise level of one x-ray. Ultimately, the authors intend to construct a detector with over one million pixels (1024 by 1024). They present the results of their development effort and various features of the design. The electronics design is discussed, with special attention to the performance requirements. The choice and design of the detective diodes, as they relate to x-ray stopping power and charge collection, are presented. An analysis of various methods of bump bonding is also presented. Finally, the authors discuss the possible need for a radiation-blocking layer, to be placed between the electronics and the detective layer, and various methods they have pursued in the construction of such a layer

  7. Bright X-ray source from a laser-driven micro-plasma-waveguide

    CERN Document Server

    Yi, Longqing

    2016-01-01

    Bright tunable x-ray sources have a number of applications in basic science, medicine and industry. The most powerful sources are synchrotrons, where relativistic electrons are circling in giant storage rings. In parallel, compact laser-plasma x-ray sources are being developed. Owing to the rapid progress in laser technology, very high-contrast femtosecond laser pulses of relativistic intensities become available. These pulses allow for interaction with micro-structured solid-density plasma without destroying the structure by parasitic pre-pulses. The high-contrast laser pulses as well as the manufacturing of materials at micro- and nano-scales open a new realm of possibilities for laser interaction with photonic materials at the relativistic intensities. Here we demonstrate, via numerical simulations, that when coupling with a readily available 1.8 Joule laser, a micro-plasma-waveguide (MPW) may serve as a novel compact x-ray source. Electrons are extracted from the walls by the laser field and form a dense ...

  8. Elasticity of Tantalum to 105 Gpa using a stress and angle-resolved x-ray diffraction

    International Nuclear Information System (INIS)

    Cynn, H; Yoo, C S

    1999-01-01

    Determining the mechanical properties such as elastic constants of metals at Mbar pressures has been a difficult task in experiment. Following the development of anisotropic elastic theory by Singh et al.[l], Mao et a1.[2] have recently developed a novel experimental technique to determine the elastic constants of Fe by using the stress and energy-dispersive x-ray diffraction (SEX). In this paper, we present an improved complementary technique, stress and angle-resolved x-ray diffraction (SAX), which we have applied to determine the elastic constants of tantalum to 105 GPa. The extrapolation of the tantalum elastic data shows an excellent agreement with the low-pressure ultrasonic data[3]. We also discuss the improvement of this SAX method over the previous SEX.[elastic constant, anisotropic elastic theory, angle-dispersive synchrotron x-ray diffraction, mechanical properties

  9. Time-resolved pump and probe x-ray absorption fine structure spectroscopy at beamline P11 at PETRA III

    Energy Technology Data Exchange (ETDEWEB)

    Göries, D., E-mail: dennis.goeries@desy.de; Roedig, P.; Stübe, N.; Meyer, J.; Warmer, M.; Weckert, E.; Meents, A., E-mail: alke.meents@desy.de [DESY Photon Science, Deutsches Elektronen-Synchrotron (DESY), Notkestraße 85, 22607 Hamburg (Germany); Dicke, B.; Naumova, M.; Rübhausen, M. [Center for Free-Electron Laser Science (CFEL), Luruper Chaussee 149, 22761 Hamburg (Germany); Galler, A.; Gawelda, W.; Geßler, P.; Sotoudi Namin, H.; Beckmann, A. [European XFEL, Albert-Einstein Ring 19, 22761 Hamburg (Germany); Britz, A.; Bressler, C. [European XFEL, Albert-Einstein Ring 19, 22761 Hamburg (Germany); The Hamburg Centre for Ultrafast Imaging, Luruper Chaussee 149, 22761 Hamburg (Germany); Schlie, M. [Institut für Experimentalphysik, University of Hamburg, Luruper Chaussee 149, 22761 Hamburg (Germany)

    2016-05-15

    We report about the development and implementation of a new setup for time-resolved X-ray absorption fine structure spectroscopy at beamline P11 utilizing the outstanding source properties of the low-emittance PETRA III synchrotron storage ring in Hamburg. Using a high intensity micrometer-sized X-ray beam in combination with two positional feedback systems, measurements were performed on the transition metal complex fac-Tris[2-phenylpyridinato-C2,N]iridium(III) also referred to as fac-Ir(ppy){sub 3}. This compound is a representative of the phosphorescent iridium(III) complexes, which play an important role in organic light emitting diode (OLED) technology. The experiment could directly prove the anticipated photoinduced charge transfer reaction. Our results further reveal that the temporal resolution of the experiment is limited by the PETRA III X-ray bunch length of ∼103 ps full width at half maximum (FWHM).

  10. Development of transient collisional excitation x-ray laser with ultra short-pulse laser

    International Nuclear Information System (INIS)

    Kado, Masataka; Kawachi, Tetsuya; Hasegawa, Noboru; Tanaka, Momoko; Sukegawa, Kouta; Nagashima, Keisuke; Kato, Yoshiaki

    2001-01-01

    We have observed lasing on Ne-like 3s-3p line from titanium (32.4 nm), Ni-like 4p-4d line from silver (13.9 nm) and tin (11.9 nm) with the transient collisional excitation (TCE) scheme that uses combination of a long pre-pulse (∼ns) and a short main pulse (∼ps). A gain coefficient of 23 cm -1 was measured for plasma length up to 4 mm with silver slab targets. We have also observed lasing on Ne-like and Ni-like lines with new TCE scheme that used pico-seconds laser pulse to generate plasma and observed strong improvement of x-ray laser gain coefficient. A gain coefficient of 14 cm -1 was measured for plasma length up to 6 mm with tin targets. (author)

  11. Review of x-ray spectroscopy from laser-produced plasmas

    International Nuclear Information System (INIS)

    Kauffman, R.L.

    1987-09-01

    Recent progress in x-ray spectroscopy from laser plasmas is reviewed. Advances in the use of K-shell spectra as a diagnostic tool is discussed. Much activity in understanding complex spectra especially from Ne I and Ni I isoelectronic series have been made. Much of the progress has been due to observation of amplification from Δn = O transitions from these configurations. The spectroscopy will be discussed and examples of spectra of the amplified lines will be shown. Finally, recent work on using x-ray spectroscopy to diagnose high density implosions will be discussed. 33 refs

  12. X-ray diffraction in laser-irradiated epsomite crystals grown in presence of borax

    International Nuclear Information System (INIS)

    Zaitseva, E.V.; Portnov, V.N.; Faddeev, M.A.; Chuprunov, E.V.

    1997-01-01

    Relative changes in the intensities ΔI/I of the (220) and (440) X-ray diffraction reflection during laser irradiation of epsomite (MgSO 2 ·7H 2 O) crystals grown from an aqueous solution in the presence of borax (Na 2 B 4 O 7 ·10H 2 O) were measured using the CoK α , CuK α , MoK α radiations. The intensities measured depend on the real crystal structure dependent on the borax content in the solution. The dependence of ΔI/I is studied as a function of borax in the solution and X-ray-radiation wavelength

  13. Ultrafast Coherent Diffraction Imaging with X-ray Free-Electron Lasers

    International Nuclear Information System (INIS)

    Chapman, H N; Bajt, S; Barty, A; Benner, W; Bogan, M; Frank, M; Hau-Riege, S; London, R; Marchesini, S; Spiller, E; Szoke, A; Woods, B; Boutet, S; Hodgson, K; Hajdu, J; Bergh, M; Burmeister, F; Caleman, C; Huldt, G; Maia, F; Seibert, M M; der Spoel, D v

    2006-01-01

    The ultrafast pulses from X-ray free-electron lasers will enable imaging of non-periodic objects at near-atomic resolution [1, Neutze]. These objects could include single molecules, protein complexes, or virus particles. The specimen would be completely destroyed by the pulse in a Coulomb explosion, but that destruction will only happen after the pulse. The scattering from the sample will give structural information about the undamaged object. There are many technical challenges that must be addressed before carrying out such experiments at an XFEL, which we are doing so with experiments at FLASH, the soft-X-ray FEL at DESY

  14. Soft x-ray microradiography and lithograph using a laser produced plasma source

    International Nuclear Information System (INIS)

    Cheng, P.C.

    1992-01-01

    Considering the hardware characteristics of the laser-induced plasma X-ray source and the limitations of the conventional cone-beam reconstruction algorithm, a general cone-beam reconstruction algorithm has been developed at our laboratory, in which the motion locus of the X-ray source is an arbitrary curve corresponding to at least a 2π continuous horizontal angular displacement in the coordinate system of the specimen. The preliminary simulation shows that the general cone-beam reconstruction algorithm consistently results in visually satisfactory images

  15. Demonstration of a transient high gain nickel-like xenon ion x-ray laser

    International Nuclear Information System (INIS)

    Lu, Peixiang; Kawachi, Tetsuya; Kishimoto, Maki

    2003-01-01

    We demonstrate a high gain nickel-like xenon ion x-ray laser using a picosecond-laser-irradiated gas puff target. The elongated x-ray laser plasma column was produced by irradiating the gas puff target with line-focused double picosecond laser pulses with a total energy of 18 J in a travelling-wave excitation scheme. Strong lasing at 9.98 nm was observed, and a high gain coefficient of 17.4 cm -1 was measured on the transient collisionally excited 4d-4p, J=0-1 transition for nickel-like xenon ion with target lengths up to 0.45 cm. A weak nickel-like lasing line at a shorter wavelength of 9.64 nm was also observed with a gain coefficient of 5.9 cm -1 . (author)

  16. Imaging ultrafast excited state pathways in transition metal complexes by X-ray transient absorption and scattering using X-ray free electron laser source

    DEFF Research Database (Denmark)

    Chen, Lin X; Shelby, Megan L; Lestrange, Patrick J

    2016-01-01

    This report will describe our recent studies of transition metal complex structural dynamics on the fs and ps time scales using an X-ray free electron laser source, Linac Coherent Light Source (LCLS). Ultrafast XANES spectra at the Ni K-edge of nickel(ii) tetramesitylporphyrin (NiTMP) were measured...... on the low-energy shoulder of the edge, which is aided by the computation of X-ray transitions for postulated excited electronic states. The observed and computed inner shell to valence orbital transition energies demonstrate and quantify the influence of the electronic configuration on specific metal...

  17. High pressure X-ray preionized TEMA-CO2 laser

    Science.gov (United States)

    Bonnie, R. J. M.; Witteman, W. J.

    1987-09-01

    The construction of a high-pressure (up to 20 atm) transversely excited CO2 laser using transverse X-ray preionization is described. High pressure operation was found to be greatly improved in comparison to UV-preionized systems. Homogeneous discharges have been achieved in the pressure range 5-20 atm, yielding a specific laser output in the order of 35 J/l.

  18. Laser-produced Au nanoparticles as X-ray contrast agents for diagnostic imaging

    Czech Academy of Sciences Publication Activity Database

    Torrisi, L.; Restuccia, N.; Cuzzocrea, S.; Paterniti, I.; Ielo, I.; Pergolizzi, S.; Cutroneo, Mariapompea; Kováčik, L.

    2017-01-01

    Roč. 50, č. 1 (2017), s. 51-60 ISSN 0017-1557 R&D Projects: GA MŠk LM2015056; GA ČR(CZ) GBP108/12/G108 Institutional support: RVO:61389005 Keywords : Au nanoparticles * Laser * X-ray diagnostic s * medical imaging * contrast medium Subject RIV: BH - Optics, Masers, Lasers OBOR OECD: Inorganic and nuclear chemistry Impact factor: 1.638, year: 2016

  19. Progress in optical-field-ionization soft x-ray lasers at LOA

    Czech Academy of Sciences Publication Activity Database

    Mocek, Tomáš; Sebban, S.; Bettaibi, I.; Zeitoun, P.; Faivre, G.; Cros, B.; Maynard, G.; Butler, A.; McKenna, C.M.; Spence, D.J.; Gonsavles, A.J.; Hooker, S.M.; Vorontsov, V.; Hallou, S.; Fajardo, M.; Kazamias, S.; Le Pape, S.; Mercere, P.; Morlens, A.S.; Valentin, C.; Balcou, P.

    2005-01-01

    Roč. 23, - (2005), s. 351-356 ISSN 0263-0346 Grant - others:EU(XE) HPRI-1999-CT-00086; EU(XE) HPMF-CT-2002-01554 Institutional research plan: CEZ:AV0Z10100523 Keywords : collisional excitation * femtosecond * guiding * high harmonic amplification * x-ray laser Subject RIV: BH - Optics, Masers, Lasers Impact factor: 2.590, year: 2005

  20. Radiation safety aspects of new X-ray free electron laser facility, SACLA

    International Nuclear Information System (INIS)

    Asano, Yoshihiro

    2013-01-01

    In the safety point of view, X-ray free electron laser facilities have some characteristics in comparison with 3 rd generation synchrotron radiation facilities. One is that the high energy electrons are always injected into the beam dump and the beamlines must be constructed in the direction of the movements of electrons, and another is that the total number of accelerated electrons of X-ray free electron laser facilities is much larger than that of synchrotron radiation facilities. In addition to the importance of safety interlock systems, therefore, it is important that high energy electrons never invade into X-ray free electron laser beamlines and the amount of accelerated electron beam losses must be reduced as much as possible. At SACLA, a safety permanent magnet was installed into the X-ray light beam axis, and a beam halo monitor and beam loss monitors were installed within and around the electron transport pipes, respectively. In comparison with the SPring-8 synchrotron radiation facility, shielding design of SACLA, outline of the radiation safety systems including the monitors will be presented

  1. X-ray laser diffraction for structure determination of the rhodopsin-arrestin complex

    Science.gov (United States)

    Zhou, X. Edward; Gao, Xiang; Barty, Anton; Kang, Yanyong; He, Yuanzheng; Liu, Wei; Ishchenko, Andrii; White, Thomas A.; Yefanov, Oleksandr; Han, Gye Won; Xu, Qingping; de Waal, Parker W.; Suino-Powell, Kelly M.; Boutet, Sébastien; Williams, Garth J.; Wang, Meitian; Li, Dianfan; Caffrey, Martin; Chapman, Henry N.; Spence, John C. H.; Fromme, Petra; Weierstall, Uwe; Stevens, Raymond C.; Cherezov, Vadim; Melcher, Karsten; Xu, H. Eric

    2016-04-01

    Serial femtosecond X-ray crystallography (SFX) using an X-ray free electron laser (XFEL) is a recent advancement in structural biology for solving crystal structures of challenging membrane proteins, including G-protein coupled receptors (GPCRs), which often only produce microcrystals. An XFEL delivers highly intense X-ray pulses of femtosecond duration short enough to enable the collection of single diffraction images before significant radiation damage to crystals sets in. Here we report the deposition of the XFEL data and provide further details on crystallization, XFEL data collection and analysis, structure determination, and the validation of the structural model. The rhodopsin-arrestin crystal structure solved with SFX represents the first near-atomic resolution structure of a GPCR-arrestin complex, provides structural insights into understanding of arrestin-mediated GPCR signaling, and demonstrates the great potential of this SFX-XFEL technology for accelerating crystal structure determination of challenging proteins and protein complexes.

  2. Reflection of femtosecond pulses from soft X-ray free-electron laser by periodical multilayers

    Energy Technology Data Exchange (ETDEWEB)

    Ksenzov, D.; Grigorian, S.; Pietsch, U. [Faculty of Physics, University of Siegen (Germany); Hendel, S.; Bienert, F.; Sacher, M.D.; Heinzmann, U. [Faculty of Physics, University of Bielefeld (Germany)

    2009-08-15

    Recent experiments on a soft X-ray free-electron laser (FEL) source (FLASH in Hamburg) have shown that multilayers (MLs) can be used as optical elements for highly intense X-ray irradiation. An effort to find most appropriate MLs has to consider the femtosecond time structure and the particular photon energy of the FEL. In this paper we have analysed the time response of 'low absorbing' MLs (e.g. such as La/B{sub 4}C) as a function of the number of periods. Interaction of a pulse train of Gaussian shaped sub-pulses using a realistic ML grown by electron-beam evaporation technique has been analysed in the soft-X-ray range. The structural parameters of the MLs were obtained by reflectivity measurements at BESSY II and subsequent profile fittings. (Abstract Copyright [2009], Wiley Periodicals, Inc.)

  3. Two-dimensional imaging detectors for structural biology with X-ray lasers.

    Science.gov (United States)

    Denes, Peter

    2014-07-17

    Our ability to harness the advances in microelectronics over the past decade(s) for X-ray detection has resulted in significant improvements in the state of the art. Biology with X-ray free-electron lasers present daunting detector challenges: all of the photons arrive at the same time, and individual high peak power pulses must be read out shot-by-shot. Direct X-ray detection in silicon pixel detectors--monolithic or hybrid--are the standard for XFELs today. For structural biology, improvements are needed for today's 10-100 Hz XFELs, and further improvements are required for tomorrow's 10+ kHz XFELs. This article will discuss detector challenges, why they arise and ways to overcome them, along with the current state of the art. © 2014 The Author(s) Published by the Royal Society. All rights reserved.

  4. Laser-produced multi-charged heavy ions as efficient soft x-ray sources

    International Nuclear Information System (INIS)

    Higashiguchi, Takeshi; Suzuki, Yuhei; Kawasaki, Masato

    2016-01-01

    We demonstrate EUV and soft x-ray sources in the 2 to 7 nm spectral region related to the beyond EUV (BEUV) question at 6x nm and a water window source based on laser-produced high-Z plasmas. Resonance emission from multiply charged ions merges to produce intense unresolved transition arrays (UTAs), extending below the carbon K edge (4.37 nm). An outline of a microscope design for single-shot live cell imaging is proposed based on a high-Z plasma UTA source, coupled to x-ray optics. We will discuss the progress and Z-scaling of UTA emission spectra to achieve lab-scale table-top, efficient, high-brightness high-Z plasma EUV-soft x-ray sources for in vivo bio-imaging applications. (author)

  5. Data processing software suite SITENNO for coherent X-ray diffraction imaging using the X-ray free-electron laser SACLA

    International Nuclear Information System (INIS)

    Sekiguchi, Yuki; Oroguchi, Tomotaka; Takayama, Yuki; Nakasako, Masayoshi

    2014-01-01

    The software suite SITENNO is developed for processing diffraction data collected in coherent X-ray diffraction imaging experiments of non-crystalline particles using an X-ray free-electron laser. Coherent X-ray diffraction imaging is a promising technique for visualizing the structures of non-crystalline particles with dimensions of micrometers to sub-micrometers. Recently, X-ray free-electron laser sources have enabled efficient experiments in the ‘diffraction before destruction’ scheme. Diffraction experiments have been conducted at SPring-8 Angstrom Compact free-electron LAser (SACLA) using the custom-made diffraction apparatus KOTOBUKI-1 and two multiport CCD detectors. In the experiments, ten thousands of single-shot diffraction patterns can be collected within several hours. Then, diffraction patterns with significant levels of intensity suitable for structural analysis must be found, direct-beam positions in diffraction patterns determined, diffraction patterns from the two CCD detectors merged, and phase-retrieval calculations for structural analyses performed. A software suite named SITENNO has been developed to semi-automatically apply the four-step processing to a huge number of diffraction data. Here, details of the algorithm used in the suite are described and the performance for approximately 9000 diffraction patterns collected from cuboid-shaped copper oxide particles reported. Using the SITENNO suite, it is possible to conduct experiments with data processing immediately after the data collection, and to characterize the size distribution and internal structures of the non-crystalline particles

  6. Low Power X-Ray Photon Resolving Imaging Array, Phase I

    Data.gov (United States)

    National Aeronautics and Space Administration — Instruments employing X-ray detection are countless, in different sectors from medicine to industry and from basic to applied science. Given this importance, and...

  7. Short-wavelength soft-x-ray laser pumped in double-pulse single-beam non-normal incidence

    International Nuclear Information System (INIS)

    Zimmer, D.; Ros, D.; Guilbaud, O.; Habib, J.; Kazamias, S.; Zielbauer, B.; Bagnoud, V.; Ecker, B.; Aurand, B.; Kuehl, T.; Hochhaus, D. C.; Neumayer, P.

    2010-01-01

    We demonstrated a 7.36 nm Ni-like samarium soft-x-ray laser, pumped by 36 J of a neodymium:glass chirped-pulse amplification laser. Double-pulse single-beam non-normal-incidence pumping was applied for efficient soft-x-ray laser generation. In this case, the applied technique included a single-optic focusing geometry for large beam diameters, a single-pass grating compressor, traveling-wave tuning capability, and an optimized high-energy laser double pulse. This scheme has the potential for even shorter-wavelength soft-x-ray laser pumping.

  8. Storage of laser pulses in a Fabry-Perot optical cavity for high flux x-ray

    International Nuclear Information System (INIS)

    Takezawa, K.; Honda, Y.; Sasao, N.; Araki, S.; Higashi, Y.; Taniguchi, T.; Urakawa, J.; Nomura, M.; Sakai, H.

    2004-01-01

    We have a plan to produce a high flux x-ray for medical use by using a Fabry-Perot optical cavity in which the lower pulses from a mode-locked laser are stored and enhanced. In this plan, the X-ray is produced from the Compton scattering of electrons in a storage ring with the laser light in the optical cavity. In order to increase X-ray flux, high power laser light is necessary. We show the enhancement of the laser power from the model locked laser with a Fabry-Perot optical cavity. (author)

  9. Characterization and control of femtosecond electron and X-ray beams at free-electron lasers

    International Nuclear Information System (INIS)

    Behrens, Christopher

    2012-11-01

    X-ray free-electron lasers (FELs) open up new frontiers in photon science, and in order to take full advantage of these unique accelerator-based light sources, the characterization and control of the femtosecond electron and X-ray beams is essential. Within this cumulative thesis, recent results achieved within the active research field of femtosecond electron and X-ray beams at FELs are reported.The basic principles of X-ray FELs are described, and concepts of longitudinal electron beam diagnostics with femtosecond accuracy are covered. Experimental results obtained with a transverse deflecting structure (TDS) and spectroscopy of coherent terahertz radiation are presented, and the suppression of coherent optical radiation effects, required for diagnostics utilizing a TDS, is demonstrated. Control of the longitudinal phase space by using multiple radio frequencies for longitudinal electron beam tailoring is presented, and a new technique of reversible electron beam heating with two TDSs is described. For the characterization of femtosecond X-ray pulses, a novel method based on dedicated longitudinal phase space diagnostics for electron beams is introduced, and recent measurements with a streaking technique using external terahertz fields are presented.

  10. Characterization and control of femtosecond electron and X-ray beams at free-electron lasers

    Energy Technology Data Exchange (ETDEWEB)

    Behrens, Christopher

    2012-11-15

    X-ray free-electron lasers (FELs) open up new frontiers in photon science, and in order to take full advantage of these unique accelerator-based light sources, the characterization and control of the femtosecond electron and X-ray beams is essential. Within this cumulative thesis, recent results achieved within the active research field of femtosecond electron and X-ray beams at FELs are reported.The basic principles of X-ray FELs are described, and concepts of longitudinal electron beam diagnostics with femtosecond accuracy are covered. Experimental results obtained with a transverse deflecting structure (TDS) and spectroscopy of coherent terahertz radiation are presented, and the suppression of coherent optical radiation effects, required for diagnostics utilizing a TDS, is demonstrated. Control of the longitudinal phase space by using multiple radio frequencies for longitudinal electron beam tailoring is presented, and a new technique of reversible electron beam heating with two TDSs is described. For the characterization of femtosecond X-ray pulses, a novel method based on dedicated longitudinal phase space diagnostics for electron beams is introduced, and recent measurements with a streaking technique using external terahertz fields are presented.

  11. Development of a hardened X-ray imager for the Megajoule Laser radiative environment

    International Nuclear Information System (INIS)

    Rousseau, A.

    2014-01-01

    Thermonuclear fusion experiments are led on Megajoule class laser facility by imploding a capsule filled with Deuterium and Tritium. In this context, it is necessary to diagnose the core size and the shape of the compressed target in order to provide valuable information and identify reasons for failure. State of the art X-ray imaging diagnostics cannot realize measurements without being perturbed by the nuclear background. The diagnostic that has been designed in this thesis combine high spatial resolution X-ray imaging at high energy and radiation tolerance to nuclear background. We have first guaranteed, theoretically and experimentally, survivability of X ray multilayer coating to energetic neutrons irradiation. Consequently, we have design the X-ray imaging system in order to achieve 5 μm resolution in a spectral range up to 95 keV. The X-ray image has then been converted into visible light in order to be easily transferred through a hardened optical relay to a protected area where the optical analyser is set. This analyser, combining light amplifier and pixelised detector, has also been studied and a novel method has been developed to reduce nuclear related transient perturbations on the device. This by parts design associated with Monte-Carlo Simulation (GEANT4) and experimental campaign on FCI facility (OMEGA) led to a coherent diagnostic architecture which will sustain high level of nuclear perturbation. (author) [fr

  12. A soft X-ray source based on a low divergence, high repetition rate ultraviolet laser

    Science.gov (United States)

    Crawford, E. A.; Hoffman, A. L.; Milroy, R. D.; Quimby, D. C.; Albrecht, G. F.

    The CORK code is utilized to evaluate the applicability of low divergence ultraviolet lasers for efficient production of soft X-rays. The use of the axial hydrodynamic code wih one ozone radial expansion to estimate radial motion and laser energy is examined. The calculation of ionization levels of the plasma and radiation rates by employing the atomic physics and radiation model included in the CORK code is described. Computations using the hydrodynamic code to determine the effect of laser intensity, spot size, and wavelength on plasma electron temperature are provided. The X-ray conversion efficiencies of the lasers are analyzed. It is observed that for a 1 GW laser power the X-ray conversion efficiency is a function of spot size, only weakly dependent on pulse length for time scales exceeding 100 psec, and better conversion efficiencies are obtained at shorter wavelengths. It is concluded that these small lasers focused to 30 micron spot sizes and 10 to the 14th W/sq cm intensities are useful sources of 1-2 keV radiation.

  13. Spin-resolved x-ray photoemission studies of ferromagnetic metals

    International Nuclear Information System (INIS)

    Klebanoff, L.E.

    1996-01-01

    Recent spin-resolved x-ray photoelectron spectroscopy (SRXPS) studies of ferromagnetic metals are reviewed. SRXPS studies of metallic Fe, Co, Co 66 Fe 4 Ni 1 B 14 Si 15 , and Ni demonstrate that core-level photoemission, and the itinerant electron response to core-hole creation, are highly spin-dependent. The exchange splitting of the Fe 2p 3/2 level is found to be 0.48±0.05 eV. Lifetime broadening results for the Fe 2p 3/2 N↑ (majority spin) and N↓ (minority spin) components indicate conservation of spin in core-hole filling processes involving the valence band. SRXPS study of the Fe 2p 3/2 peak asymmetry α reveals a dependence of electron endash hole excitation on the spin of the core hole. Spin analysis of the Fe 3s XPS line shape shows it to be a three-component spectrum, rather than the two-component line shape assumed previously. A photon energy dependence of one of the Fe 3s components explains disagreement among previous Fe 3s XPS results. Comparisons of SRXPS from Co metal and Co 66 Fe 4 Ni 1 B 14 Si 15 directly demonstrate the effect of a reduced atomic magnetic moment on the spin dependence of core-level XPS. The behavior of lifetime broadenings for the N↑ and N↓ Co 2p 3/2 components show that the reduced Co magnetic moment found in the Co 66 Fe 4 Ni 1 B 14 Si 15 amorphous glass is due to the transfer of ↑-spin valence electron density to the ↓-spin valence band upon glass formation. SRXPS also allows investigation of spin-dependent core-hole screening processes and satellite production, as demonstrated in SRXPS studies of ferromagnetic Ni. Future directions of SRXPS are also explored. copyright 1996 American Vacuum Society

  14. Interferometric studies of laser-created plasmas using compact soft x-ray lasers

    International Nuclear Information System (INIS)

    Dunn, J; Nilsen, J; Moon, S; Keenan, R; Jankowska, E; Maconi, M C; Hammarsten, E C; Filevich, J; Hunter, J R; Smith, R F; Shlyaptsev, V; Rocca, J J

    2003-01-01

    We summarize results of several successful dense plasma diagnostics experiments realized by combining two different kinds of table-top soft x-ray lasers with an amplitude division interferometer based on diffraction grating beam splitters. In the first set of experiments this robust high throughput diffraction grating interferometer (DGI) was used with a 46.9 nm portable capillary discharge laser to study the dynamics of line focus and point focus laser-created plasmas. The measured electron density profiles, which differ significantly from those expected from a classical expansion, unveil important two-dimensional effects of the dynamics of these plasmas. A second DGI customized to operate in combination with a 14.7 nm Ni-like Pd transient gain laser was used to perform interferometry of line focus laser-created plasmas with picosecond time resolution. These measurements provide valuable new benchmarks for complex hydrodynamic codes and help bring new understanding of the dynamics of dense plasmas. The instrumentation and methodology we describe is scalable to significantly shorter wavelengths, and constitutes a promising scheme for extending interferometry to the study of very dense plasmas such as those investigated for inertial confinement fusion

  15. Prospects for compact high-intensity laser synchrotron x-ray and gamma sources

    International Nuclear Information System (INIS)

    Pogorelsky, I.V.

    1996-11-01

    A laser interacting with a relativistic electron beam behaves like a virtual wiggler of an extremely short period equal to half of the laser wavelength. This approach opens a route to relatively compact, high-brightness x-ray sources alternative or complementary to conventional synchrotron light sources. Although not new, the laser synchrotron source (LSS) concept is still waiting for a convincing demonstration. Available at the BNL Accelerator Test Facility (ATF), a high-brightness electron beam and the high-power CO 2 laser may be used as prototype LSS brick stones. In a feasible demonstration experiment, 10-GW, 100-ps CO 2 laser beam will be brought to a head-on collision with a 10-ps, 0.5-nC, 50 MeV electron bunch. Flashes of collimated 4.7 keV (2.6 angstrom) x-rays of 10-ps pulse duration, with a flux of ∼ 10 19 photons/sec, will be produced via linear Compton backscattering. The x-ray spectrum is tunable proportionally to the e-beam energy. A rational short-term extension of the proposed experiment would be further enhancement of the x-ray flux to the 10 22 photons/sec level, after the ongoing ATF CO 2 laser upgrade to 5 TW peak power and electron bunch shortening to 3 ps is realized. In the future, exploiting the promising approach of a high-gradient laser wake field accelerator, a compact ''table-top'' LSS of monochromatic gamma radiation may become feasible

  16. Prospects for compact high-intensity laser synchrotron x-ray and gamma sources

    International Nuclear Information System (INIS)

    Pogorelsky, I.V.

    1997-01-01

    A laser interacting with a relativistic electron beam behaves like a virtual wiggler of an extremely short period equal to half of the laser wavelength. This approach opens a route to relatively compact, high- brightness x-ray sources alternative or complementary to conventional synchrotron light sources. Although not new, the laser synchrotron source (LSS) concept is still waiting for a convincing demonstration. Available at the BNL Accelerator Test Facility (ATF), a high- brightness electron beam and the high-power C0 2 laser may be used as prototype LSS brick stones. In a feasible demonstration experiment, 10 GW, 100 ps C0 2 laser beam will be brought to a head-on collision with a 10 ps, 0.5 nC, 50 MeV electron bunch. Flashes of collimated 4.7 keV (2.6 A) x-rays of 10-ps pulse duration, with a flux of ∼10 19 photons/sec, will be produced via linear Compton backscattering. The x-ray spectra is tunable proportionally to the e- beam energy. A rational short-term extension of the proposed experiment would be further enhancement of the x-ray flux to the 10 22 photon/sec level, after the ongoing ATF C0 2 laser upgrade to 5 TW peak power and electron bunch shortening to 3 ps is realized. In the future, exploiting the promising approach of a high-gradient laser wake field accelerator, a compact ''table- top'' LSS of monochromatic gamma radiation may become feasible

  17. Soft x-ray free-electron laser induced damage to inorganic scintillators

    Czech Academy of Sciences Publication Activity Database

    Burian, Tomáš; Hájková, Věra; Chalupský, Jaromír; Vyšín, Luděk; Boháček, Pavel; Přeček, Martin; Wild, J.; Özkan, C.; Coppola, N.; Farahani, S.D.; Schulz, J.; Sinn, H.; Tschentscher, T.; Gaudin, J.; Bajt, S.; Tiedtke, K.; Toleikis, S.; Chapman, H.N.; Loch, R.A.; Jurek, M.; Sobierajski, R.; Krzywinski, J.; Moeller, S.; Harmand, M.; Galasso, G.; Nagasono, M.; Saskl, K.; Sovák, P.; Juha, Libor

    2015-01-01

    Roč. 5, č. 2 (2015), 254-264 ISSN 2159-3930 R&D Projects: GA ČR(CZ) GAP108/11/1312; GA MŠk EE2.3.30.0057 Grant - others:OP VK 4 POSTDOK(XE) CZ.1.07/2.3.00/30.0057 Institutional support: RVO:68378271 Keywords : fluorescent and luminescent materials * laser damage * free-electron lasers * soft x-rays * laser materials processing Subject RIV: BH - Optics, Masers, Lasers Impact factor: 2.657, year: 2015

  18. Advanced design and modeling concepts for recombination x-ray lasers

    International Nuclear Information System (INIS)

    Eder, D.C.; Rosen, M.D.; Shephard, R.; Staffin, R.; Nash, J.K.; Keane, C.J.

    1990-01-01

    Geometric, kinetic, and trapping issues, in short and ultrashort recombination x-ray lasers, are discussed. The design of a composite target consisting of a lasant strip on a plastic backing is described. Examples of modeling showing the effect of photon trapping and uncertainties in other physical processes on calculated gain coefficients are given. A simple and accurate expression for photon trapping in cylindrical geometry is presented. Recombination lasers that have the ground state as the lower laser state are shown to have small I sat 's and corresponding low efficiencies. Scaling laws for femtosecond laser-plasma interactions are presented. 19 refs

  19. Bond Shortening (1.4 Å) in the Singlet and Triplet Excited States of [Ir2(dimen)4]2+ in Solution Determined by Time-Resolved X-ray Scattering

    DEFF Research Database (Denmark)

    Haldrup, Martin Kristoffer; Harlang, Tobias; Christensen, Morten

    2011-01-01

    Ground- and excited-state structures of the bimetallic, ligand-bridged compound Ir2(dimen)42+ are investigated in acetonitrile by means of time-resolved X-ray scattering. Following excitation by 2 ps laser pulses at 390 nm, analysis of difference scattering patterns obtained at eight different ti...

  20. Investigation of the interaction of high intensity laser light with solids and hot plasma using X-ray spectroscopic technique

    International Nuclear Information System (INIS)

    Zigler, A.

    1978-06-01

    This work investigates the properties of high power laser-produced plasmas by developing and applying x-ray spectroscopic methods which utilize spatial resolution. The shadow techniques which were developed in this work yield a high spatial resolution of 5-15μm together with an adequate X-ray spectral resolution for single shots of laser power flux of 2.10 13 W/cm -2 . The intensity distribution in the source is calculated from the partial shadow by numerical differentiation. The main advantage of the present method is the ability to obtain spatial information simultaneously for strong and weak spectral lines for a single shot of medium power laser. Plasma parameters were derived from H-like and He-like lines and their inner-shell satellites, which were obtained from Mg, Al and Si targets. Using shadow techniques, the sizes of the emitting regions of the various spectral lines were measured; the spatial variation of the ionization stage, the electron temperature and density were investigated. A constant electron temperature of (250+-50)eV and electron density scale-length of about 50μm were derived for an expanding plasma. An experimental investigation of the possible origin and the mechanisms responsible for the Ksub(α) radiation in laser-produced plasma was carried out. It is shown that the Ksub(α) radiation was generated by fast suprathermal electrons and originated inside the target behind the interaction zone of the shock and heat waves. Energy penetration depth and hot plasma expansion were tested by using multilayer targets, thin foils and achieving a two-dimensional spatially resolved X-ray Al spectrum. (B.G.)

  1. Soft x-ray power diagnostic improvements at the Omega Laser Facility

    International Nuclear Information System (INIS)

    Sorce, C.; Schein, J.; Weber, F.; Widmann, K.; Campbell, K.; Dewald, E.; Turner, R.; Landen, O.; Jacoby, K.; Torres, P.; Pellinen, D.

    2006-01-01

    Soft x-ray power diagnostics are essential for evaluating high temperature laser plasma experiments. The Dante soft x-ray spectrometer, a core diagnostic for radiation flux and temperature measurements of Hohlraums, installed on the Omega Laser Facility at the Laboratory for Laser Energetics has recently undergone a series of upgrades. Work performed at Brookhaven National Laboratory for the development of the National Ignition Facility (NIF) Dante spectrometer enables the Omega Dante to offer a total of 18 absolutely calibrated channels in the energy range from 50 eV to 20 keV. This feature provides Dante with the capability to measure higher, NIF relevant, radiation temperatures with increased accuracy including a differentiation of higher energy radiation such as the Au M and L bands. Diagnostic monitoring using experimental data from directly driven Au spherical shots is discussed

  2. Fabrication of the multilayer beam splitters with large area for soft X-ray laser interferometer

    International Nuclear Information System (INIS)

    Wang Zhanshan; Zhang Zhong; Wang Fengli; Wu Wenjuan; Wang Hongchang; Qin Shuji; Chen Lingyan

    2004-01-01

    The soft X-ray laser Mach-Zehnder interferometer is an important tool to measure the electron densities of a laser-produced plasma near the critical surface. The design of a multilayer beam splitter at 13.9 nm for soft X-ray laser Mach-Zehnder interferometer is completed based on the standard of maximizing product of reflectivity and transmission of the beam splitter. The beam splitters which is Mo/Si multilayers on 10 mm x 10 mm area Si 3 N 4 membrane are fabricated using the magnetron sputtering. The figure error of the beam splitter has reached the deep nanometer magnitude by using optical profiler and the product of reflectivity and transmission measured by synchrotron radiation is up to to 4%. (authors)

  3. Design of the nickel-like tin x-ray laser at 12.0 nm

    International Nuclear Information System (INIS)

    Yan Fei; Zhang Jie; Lu Xin; Zhong, Jia Y.

    2005-01-01

    The effects of the drive laser intensity, pulse duration, and pulse configuration on the performance of the Ni-like Sn x-ray laser at 12.0 nm (4d→4p, J=0→1) are investigated with use of a one-dimensional hydrodynamic code coupled with an atomic physics code. High gain operation is predicted for the optimized drive pulse configuration. The effects of refraction and saturation on the propagation of the x-ray laser in the plasma medium are also investigated by use of a two-dimensional ray-tracing code. The results show that the refraction plays an important role. The saturated output with an effective gain product length of 17.88 can be obtained for an ∼0.40-cm-long plasma column by use of optimized parameters

  4. Multicascade X-Ray Free-Electron Laser with Harmonic Multiplier and Two-Frequency Undulator

    Science.gov (United States)

    Zhukovsky, K. V.

    2018-06-01

    The feasibility of generation of powerful x-ray radiation by a cascade free-electron laser (FEL) with amplification of higher harmonics using a two-frequency undulator is studied. To analyze the FEL operation, a complex phenomenological single-pass FEL model is developed and used. It describes linear and nonlinear generation of harmonics in the FEL with seed laser that takes into account initial electron beam noise and describes all main losses of each harmonic in each FEL cascade. The model is also calibrated against and approved by the experimental FEL data and available results of three-dimensional numerical simulation. The electron beam in the undulator is assumed to be matched and focused, and the dynamics of power in the singlepass FEL with cascade harmonic multipliers is investigated to obtain x-ray laser radiation in the FEL having the shortest length, beam energy, and frequency of the seed laser as low as possible. In this context, the advantages of the two-frequency undulator used for generation of harmonics are demonstrated. The evolution of harmonics in a multicascade FEL with multiplication of harmonics is investigated. The operation of the cascade FEL at the wavelength λ = 1.14 nm, generating 30 MW already on 38 m with the seed laser operating at a wavelength of 11.43 nm corresponding to the maximal reflectivity of the multilayered mirror MoRu/Be coating is investigated. In addition, the operation of the multicascade FEL with accessible seed UVlaser operating at a wavelength of 157 nm (F2 excimer UV-laser) and electron beam with energy of 0.5 GeV is investigated. X-ray radiation simulated in it at the wavelength λ 3.9 nm reaches power of 50 MW already at 27 m, which is by two orders of magnitude shorter than 3.4 km of the x-ray FEL recently put into operation in Europe.

  5. Single mimivirus particles intercepted and imaged with an X-ray laser

    Science.gov (United States)

    Seibert, M. Marvin; Ekeberg, Tomas; Maia, Filipe R. N. C.; Svenda, Martin; Andreasson, Jakob; Jönsson, Olof; Odić, Duško; Iwan, Bianca; Rocker, Andrea; Westphal, Daniel; Hantke, Max; DePonte, Daniel P.; Barty, Anton; Schulz, Joachim; Gumprecht, Lars; Coppola, Nicola; Aquila, Andrew; Liang, Mengning; White, Thomas A.; Martin, Andrew; Caleman, Carl; Stern, Stephan; Abergel, Chantal; Seltzer, Virginie; Claverie, Jean-Michel; Bostedt, Christoph; Bozek, John D.; Boutet, Sébastien; Miahnahri, A. Alan; Messerschmidt, Marc; Krzywinski, Jacek; Williams, Garth; Hodgson, Keith O.; Bogan, Michael J.; Hampton, Christina Y.; Sierra, Raymond G.; Starodub, Dmitri; Andersson, Inger; Bajt, Saša; Barthelmess, Miriam; Spence, John C. H.; Fromme, Petra; Weierstall, Uwe; Kirian, Richard; Hunter, Mark; Doak, R. Bruce; Marchesini, Stefano; Hau-Riege, Stefan P.; Frank, Matthias; Shoeman, Robert L.; Lomb, Lukas; Epp, Sascha W.; Hartmann, Robert; Rolles, Daniel; Rudenko, Artem; Schmidt, Carlo; Foucar, Lutz; Kimmel, Nils; Holl, Peter; Rudek, Benedikt; Erk, Benjamin; Hömke, André; Reich, Christian; Pietschner, Daniel; Weidenspointner, Georg; Strüder, Lothar; Hauser, Günter; Gorke, Hubert; Ullrich, Joachim; Schlichting, Ilme; Herrmann, Sven; Schaller, Gerhard; Schopper, Florian; Soltau, Heike; Kühnel, Kai-Uwe; Andritschke, Robert; Schröter, Claus-Dieter; Krasniqi, Faton; Bott, Mario; Schorb, Sebastian; Rupp, Daniela; Adolph, Marcus; Gorkhover, Tais; Hirsemann, Helmut; Potdevin, Guillaume; Graafsma, Heinz; Nilsson, Björn; Chapman, Henry N.; Hajdu, Janos

    2014-01-01

    X-ray lasers offer new capabilities in understanding the structure of biological systems, complex materials and matter under extreme conditions1–4. Very short and extremely bright, coherent X-ray pulses can be used to outrun key damage processes and obtain a single diffraction pattern from a large macromolecule, a virus or a cell before the sample explodes and turns into plasma1. The continuous diffraction pattern of non-crystalline objects permits oversampling and direct phase retrieval2. Here we show that high-quality diffraction data can be obtained with a single X-ray pulse from a non-crystalline biological sample, a single mimivirus particle, which was injected into the pulsed beam of a hard-X-ray free-electron laser, the Linac Coherent Light Source5. Calculations indicate that the energy deposited into the virus by the pulse heated the particle to over 100,000 K after the pulse had left the sample. The reconstructed exit wavefront (image) yielded 32-nm full-period resolution in a single exposure and showed no measurable damage. The reconstruction indicates inhomogeneous arrangement of dense material inside the virion. We expect that significantly higher resolutions will be achieved in such experiments with shorter and brighter photon pulses focused to a smaller area. The resolution in such experiments can be further extended for samples available in multiple identical copies. PMID:21293374

  6. First set of gated x-ray imaging diagnostics for the Laser Megajoule facility

    Energy Technology Data Exchange (ETDEWEB)

    Rosch, R.; Trosseille, C.; Caillaud, T.; Allouche, V.; Bourgade, J. L.; Briat, M.; Brunel, P.; Burillo, M.; Casner, A.; Depierreux, S.; Gontier, D.; Jadaud, J. P.; Le Breton, J. P.; Llavador, P.; Loupias, B.; Miquel, J. L.; Oudot, G.; Perez, S.; Raimbourg, J.; Rousseau, A. [CEA-DAM Ile de France, Bruyères-le-Châtel, 91297 Arpajon Cedex (France); and others

    2016-03-15

    The Laser Megajoule (LMJ) facility located at CEA/CESTA started to operate in the early 2014 with two quadruplets (20 kJ at 351 nm) focused on target for the first experimental campaign. We present here the first set of gated x-ray imaging (GXI) diagnostics implemented on LMJ since mid-2014. This set consists of two imaging diagnostics with spatial, temporal, and broadband spectral resolution. These diagnostics will give basic measurements, during the entire life of the facility, such as position, structure, and balance of beams, but they will also be used to characterize gas filled target implosion symmetry and timing, to study x-ray radiography and hydrodynamic instabilities. The design requires a vulnerability approach, because components will operate in a harsh environment induced by neutron fluxes, gamma rays, debris, and shrapnel. Grazing incidence x-ray microscopes are fielded as far as possible away from the target to minimize potential damage and signal noise due to these sources. These imaging diagnostics incorporate microscopes with large source-to-optic distance and large size gated microchannel plate detectors. Microscopes include optics with grazing incidence mirrors, pinholes, and refractive lenses. Spatial, temporal, and spectral performances have been measured on x-ray tubes and UV lasers at CEA-DIF and at Physikalisch-Technische Bundesanstalt BESSY II synchrotron prior to be set on LMJ. GXI-1 and GXI-2 designs, metrology, and first experiments on LMJ are presented here.

  7. Analysis of neon soft x-ray spectra from short-pulse laser-produced plasmas

    International Nuclear Information System (INIS)

    Abare, A.C.; Keane, C.J.; Crane, J.K.; DaSilva, L.B.; Lee, R.W.; Perry, M.D.; Falcone, R.W.

    1993-04-01

    We report preliminary results from the analysis of streaked soft x-ray neon spectra a gas jet target. In obtained from the interaction of a picosecond Nd:glass laser with these experiments streaked spectra show prompt harmonic emission followed by longer time duration soft x-ray line emission. The majority of the line emission observed was found to originate from Li- and Be-like Ne and the major transitions in the observed spectra have been identified. Li-like emission lines were observed to decay faster in time than Be-like transitions, suggesting that recombination is taking place. Line ratios of n=4-2 and n=3-2 transitions supported the view that these lines were optically thin and thick, respectively. The time history of Li-like Ne 2p-4d and 2p-3d lines is in good agreement with a simple adiabatic expansion model coupled to a time dependent collisional-radiative code. Further x-ray spectroscopic analysis is underway which is aimed at diagnosing plasma conditions and assessing the potential of this recombining neon plasma as a quasi-steady-state recombination x-ray laser medium

  8. Bent crystal X-ray optics for the diagnosis and applications of laser-produced plasmas

    International Nuclear Information System (INIS)

    Loetzsch, Robert

    2012-01-01

    The present thesis discussed several aspects of X-ray optics based on bent crystals and a number of applications of these optics. First, a deeper insight into the reflection properties of elastically bent perfect crystal optics was gained by the consideration of all deformation effects. It was shown that the reflection properties depend on the lateral position on the crystal, an effect that was not addressed before, neither experimentally nor theoretically. To investigate this effect, an apparatus for the measurement of Bragg angles of bent crystals with high angular resolution was built. It was measured that the lattice plane distances of two-dimensionally bent crystals vary laterally by up to 10 -4 . This effect has to be considered in high resolution X-ray spectroscopy and imaging with these bent crystals. It can explain discrepancies in theoretical and experimental spectrometer resolution with spherically bent crystals. Besides these principal investigations, in this thesis a number of X-ray optics were presented that demonstrate the application potential of bent crystal optics. This includes two optics that are used in the field of applications of laser-produced plasmas as high repeating hard X-ray sources. It was shown that an X-ray spectrometer based on full cylinder rings of highly oriented pyrolytic graphite is capable to record the rather weak single shot pulses from a high repeating 1 er-plasma X-ray source. This is possible due to the high collection efficiency of the instrument of up to 5.10 -4 . Furthermore, X-ray optics based on toroidally bent crystals that make it possible to spectrally select a bandwidth of ∝1 eV and focus the ultrashort X-ray pulses from such a laser-plasma source, were designed, prepared and characterized. It was shown that these bent crystals provide the calculated integrated reflectivity, the predicted bandwidth and focus to spot sizes smaller than 60 μm. A novel application of toroidally bent crystals was pointed out: a

  9. Time resolved, 2-D hard X-ray imaging of relativistic electron-beam target interactions on ETA-II

    International Nuclear Information System (INIS)

    Crist, C.E.; Sampayan, S.; Westenskow, G.; Caporaso, G.; Houck, T.; Weir, J.; Trimble, D.; Krogh, M.

    1998-01-01

    Advanced radiographic applications require a constant source size less than 1 mm. To study the time history of a relativistic electron beam as it interacts with a bremsstrahlung converter, one of the diagnostics they use is a multi-frame time-resolved hard x-ray camera. They are performing experiments on the ETA-II accelerator at Lawrence Livermore National Laboratory to investigate details of the electron beam/converter interactions. The camera they are using contains 6 time-resolved images, each image is a 5 ns frame. By starting each successive frame 10 ns after the previous frame, they create a 6-frame movie from the hard x-rays produced from the interaction of the 50-ns electron beam pulse

  10. Phased-Resolved Strain Measuremetns in Hydrated Ordinary Portland Cement Using Synchrotron x-Rays (Prop. 2003-033)

    International Nuclear Information System (INIS)

    Biernacki, Joseph J.; Watkins, Thomas R.; Parnham, C.J.; Hubbard, Camden R.; Bai, J.

    2006-01-01

    X-ray diffraction methods developed for the determination of residual stress states in crystalline materials have been applied to study residual strains and strains because of mechanical loading of ordinary portland cement paste. Synchrotron X-rays were used to make in situ measurements of interplanar spacings in the calcium hydroxide (CH) phase of hydrated neat portland cement under uniaxial compression. The results indicate that strains on the order of 1/100 000 can be resolved providing an essentially new technique by which to measure the phase-resolved meso-scale mechanical behavior of cement under different loading conditions. Evaluation of these strain data in view of published elastic parameters for CH suggests that the CH carries a large fraction of the applied stress and that plastic interactions with the matrix are notable.

  11. Streaked, x-ray-transmission-grating spectrometer

    International Nuclear Information System (INIS)

    Ceglio, N.M.; Roth, M.; Hawryluk, A.M.

    1981-08-01

    A free standing x-ray transmission grating has been coupled with a soft x-ray streak camera to produce a time resolved x-ray spectrometer. The instrument has a temporal resolution of approx. 20 psec, is capable of covering a broad spectral range, 2 to 120 A, has high sensitivity, and is simple to use requiring no complex alignment procedure. In recent laser fusion experiments the spectrometer successfully recorded time resolved spectra over the range 10 to 120 A with a spectral resolving power, lambda/Δlambda of 4 to 50, limited primarily by source size and collimation effects

  12. Resolving the Origin of the Diffuse Soft X-ray Background

    Science.gov (United States)

    Smith, Randall K.; Foster, Adam R.; Edgar, Ricard J.; Brickhouse, Nancy S.; Sanders, Wilton T.

    2012-01-01

    In January 1993, the Diffuse X-ray Spectrometer (DXS) measured the first high-resolution spectrum of the diffuse soft X-ray background between 44-80A. A line-dominated spectrum characteristic of a 10(exp 6)K collisionally ionized plasma' was expected but while the observed spectrum was clearly line-dominated, no model would fit. Then in 2003 the Cosmic Hot Interstellar Plasma Spectrometer (CHIPS) launched and observed the diffuse extreme-ultraviolet (EUV) spectrum between 90- 265A. Although many emission lines were again expected; only Fe IX at 171.1A was detected. The discovery of X-rays from comets led to the realization that heavy ions (Z=6-28) in the solar wind will emit soft X-rays as the ions interact via charge exchange with neutral atoms in the heliosphere and geocorona. Using a new model for solar wind charge exchange (SWCX) emission, we show that the diffuse soft X-ray background can be understood as a combination of emission from charge exchange onto the slow and fast solar wind together with a more distant and diffuse hot (10(exp 6)K) plasma.

  13. Highly lead-loaded red plastic scintillators as an X-ray imaging system for the laser Mega Joule

    International Nuclear Information System (INIS)

    Hamel, Matthieu; Normand, Stephane; Turk, Gregory; Darbon, Stephane

    2012-01-01

    The scope of this project intends to record spatially resolved images of core shape and size of a deuterium-tritium micro-balloon during inertial confinement fusion (ICF) experiments at Laser Mega Joule facility (LMJ). We need to develop an x-ray imaging system which can operate in the hard radiative background generated by an ignition shot of ICF. The scintillator is a part of the imaging system and has to gather a compromise of scintillating properties (scintillating efficiency, decay time, emission wavelength) so as to both operate in the hard radiative environment and to allow the acquisition of spatially resolved images. Inorganic scintillators cannot be used because no compromise can be found regarding the expected scintillating properties. Most of them are not fast enough and emit blue light. Organic scintillators are generally fast, but present low x-ray photoelectric absorption in the 10 to 40 keV range. This does not enable the acquisition of spatially resolved images. To this aim, we have developed highly lead-loaded and red-fluorescent fast plastic scintillators. Such a combination is not currently available via scintillator suppliers, since they propose only blue-fluorescent plastic scintillators doped with up to 12 wt% Pb. Thus, incorporation ratio up to 27 wt% Pb has been reached in our laboratory, which can afford a plastic scintillator with an outstanding Z(eff) close to 50. X-rays in the 10 to 40 keV range can thus interact with a higher probability of photoelectric effect than for classic organic scintillators, such as NE-102. The strong orange-red fluorescence can be filtered, so that we can eliminate residual Cerenkov light, generated by gamma-ray absorption in glass parts of the imaging system. Characteristic decay times of our scintillators evaluated under UV excitation were estimated to be in the range 10 to 13 ns. (authors)

  14. Applications of a table-top time-resolved luminescence spectrometer with nanosecond soft X-ray pulse excitation

    Czech Academy of Sciences Publication Activity Database

    Brůža, P.; Pánek, D.; Fidler, V.; Benedikt, P.; Čuba, V.; Gbur, T.; Boháček, Pavel; Nikl, Martin

    2014-01-01

    Roč. 61, č. 1 (2014), s. 448-451 ISSN 0018-9499 R&D Projects: GA ČR GA13-09876S Institutional support: RVO:68378271 Keywords : LiCaAlF 6 * luminescence * scintillators * soft x-ray * SrHfO 3 * time-resolved spectroscopy * ZnO :Ga Subject RIV: BM - Solid Matter Physics ; Magnetism Impact factor: 1.283, year: 2014

  15. Time-resolved x-ray diffraction measurement of C60 under high pressure and temperature using synchrotron radiation

    International Nuclear Information System (INIS)

    Horikawa, T; Suito, K; Kobayashi, M; Onodera, A

    2002-01-01

    C 60 has been studied by means of time-resolved x-ray diffraction measurements using synchrotron radiation. Diffraction patterns were recorded at intervals of 1-10 min for samples under high pressure (12.5 and 14.3 GPa) and high temperature (up to 800 deg. C) for, at the longest, 3 h. Time, pressure, and temperature dependences of the C 60 structure are presented and the relevance to the hardness of materials derived from C 60 is discussed

  16. DNA strand breaks induced by soft X-ray pulses from a compact laser plasma source

    Science.gov (United States)

    Adjei, Daniel; Wiechec, Anna; Wachulak, Przemyslaw; Ayele, Mesfin Getachew; Lekki, Janusz; Kwiatek, Wojciech M.; Bartnik, Andrzej; Davídková, Marie; Vyšín, Luděk; Juha, Libor; Pina, Ladislav; Fiedorowicz, Henryk

    2016-03-01

    Application of a compact laser plasma source of soft X-rays in radiobiology studies is demonstrated. The source is based on a laser produced plasma as a result of irradiation of a double-stream gas puff target with nanosecond laser pulses from a commercially available Nd:YAG laser. The source allows irradiation of samples with soft X-ray pulses in the "water window" spectral range (wavelength: 2.3-4.4 nm; photon energy: 280-560 eV) in vacuum or a helium atmosphere at very high-dose rates and doses exceeding the kGy level. Single-strand breaks (SSB) and double-strand breaks (DBS) induced in DNA plasmids pBR322 and pUC19 have been measured. The different conformations of the plasmid DNA were separated by agarose gel electrophoresis. An exponential decrease in the supercoiled form with an increase in linear and relaxed forms of the plasmids has been observed as a function of increasing photon fluence. Significant difference between SSB and DSB in case of wet and dry samples was observed that is connected with the production of free radicals in the wet sample by soft X-ray photons and subsequent affecting the plasmid DNA. Therefore, the new source was validated to be useful for radiobiology experiments.

  17. Catalysts at work: From integral to spatially resolved X-ray absorption spectroscopy

    DEFF Research Database (Denmark)

    Grunwaldt, Jan-Dierk; Kimmerle, B.; Baiker, A.

    2009-01-01

    available techniques, X-ray absorption spectroscopy (XAS) is a well-suited tool for this purpose as the different selected examples highlight. Two different techniques, scanning and full-field X-ray microscopy/tomography, are described and compared. At first, the tomographic structure of impregnated alumina...... pellets is presented using full-field transmission microtomography and compared to the results obtained with a scanning X-ray microbeam technique to analyse the catalyst bed inside a catalytic quartz glass reactor. On the other hand, by using XAS in scanning microtomography, the structure...... metal-based catalysts. In order to obtain spectroscopic information on the spatial variation of the oxidation state of the catalyst inside the reactor XAS spectra were recorded by scanning with a micro-focussed beam along the catalyst bed. Alternatively, full-field transmission imaging was used...

  18. Resolving the origin of the diffuse soft X-ray background

    Energy Technology Data Exchange (ETDEWEB)

    Smith, Randall K.; Foster, Adam R.; Edgar, Richard J.; Brickhouse, Nancy S. [Harvard-Smithsonian Center for Astrophysics, 60 Garden Street, Cambridge MA 02138 (United States)

    2014-05-20

    The ubiquitous diffuse soft (1/4 keV) X-ray background was one of the earliest discoveries of X-ray astronomy. At least some of the emission may arise from charge exchange between solar wind ions and neutral atoms in the heliosphere, but no detailed models have been fit to the available data. Here, we report on a new model for charge exchange in the solar wind, which, when combined with a diffuse hot plasma component, filling the Local Cavity provides a good fit to the only available high-resolution soft X-ray and extreme ultraviolet spectra using plausible parameters for the solar wind. The implied hot plasma component is in pressure equilibrium with the local cloud that surrounds the solar system, creating for the first time a self-consistent picture of the local interstellar medium.

  19. Measurements of laser generated soft X-ray emission from irradiated gold foils

    Energy Technology Data Exchange (ETDEWEB)

    Davis, J. S.; Keiter, P. A.; Klein, S. R.; Drake, R. P.; Shvarts, D. [University of Michigan, 2455 Hayward St., Ann Arbor, Michigan 48109 (United States); Frank, Y.; Raicher, E.; Fraenkel, M. [Soreq Nuclear Research Center, Yavne (Israel)

    2016-11-15

    Soft x-ray emission from laser irradiated gold foils was measured at the Omega-60 laser system using the Dante photodiode array. The foils were heated with 2 kJ, 6 ns laser pulses and foil thicknesses were varied between 0.5, 1.0, and 2.0 μm. Initial Dante analysis indicates peak emission temperatures of roughly 100 eV and 80 eV for the 0.5 μm and 1.0 μm thick foils, respectively, with little measurable emission from the 2.0 μm foils.

  20. Spot size characterization of focused non-Gaussian X-ray laser beams

    Czech Academy of Sciences Publication Activity Database

    Chalupský, Jaromír; Krzywinski, J.; Juha, Libor; Hájková, Věra; Cihelka, Jaroslav; Burian, Tomáš; Vyšín, Luděk; Gaudin, J.; Gleeson, A.; Jurek, M.; Khorsand, A.R.; Klinger, D.; Wabnitz, H.; Sobierajski, R.; Störmer, M.; Tiedtke, K.; Toleikis, S.

    2010-01-01

    Roč. 18, č. 26 (2010), s. 27836-27845 ISSN 1094-4087 R&D Projects: GA AV ČR KAN300100702; GA MŠk LC510; GA MŠk(CZ) LC528; GA ČR GAP208/10/2302; GA MŠk LA08024; GA AV ČR IAAX00100903; GA MŠk(CZ) ME10046 Institutional research plan: CEZ:AV0Z10100523 Keywords : X-ray laser * free-electron laser * beam characterization * ablation Subject RIV: BH - Optics, Masers, Lasers Impact factor: 3.749, year: 2010

  1. Plasma-based X-ray laser at 21 nm for multidisciplinary applications

    Czech Academy of Sciences Publication Activity Database

    Mocek, Tomáš; Rus, Bedřich; Kozlová, Michaela; Polan, Jiří; Homer, Pavel; Jakubczak, Krzysztof; Stupka, Michal; Snopek, David; Nejdl, Jaroslav; Edwards, M.H.; Whittaker, D.S.; Tallents, G. J.; Mistry, P.; Pert, G. J.; Booth, N.; Zhai, Z.; Fajardo, M.; Zeitoun, P.; Chalupský, Jaromír; Hájková, Věra; Juha, Libor

    2009-01-01

    Roč. 54, č. 2 (2009), s. 439-444 ISSN 1434-6060 R&D Projects: GA AV ČR KAN300100702; GA ČR GA202/05/2316; GA MŠk(CZ) LC528; GA ČR GC202/07/J008; GA MŠk(CZ) 7E08094; GA MŠk(CZ) 7E09092 EU Projects: European Commission(XE) 506350 - LASERLAB-EUROPE Institutional research plan: CEZ:AV0Z10100523 Keywords : x-ray laser * laser ablation * microstruturing * dense plasma probing Subject RIV: BH - Optics, Masers, Lasers Impact factor: 1.420, year: 2009

  2. Three dimensional characterization of laser ablation craters using high resolution X-ray computed tomography

    Science.gov (United States)

    Galmed, A. H.; du Plessis, A.; le Roux, S. G.; Hartnick, E.; Von Bergmann, H.; Maaza, M.

    2018-01-01

    Laboratory X-ray computed tomography is an emerging technology for the 3D characterization and dimensional analysis of many types of materials. In this work we demonstrate the usefulness of this characterization method for the full three dimensional analysis of laser ablation craters, in the context of a laser induced breakdown spectroscopy setup. Laser induced breakdown spectroscopy relies on laser ablation for sampling the material of interest. We demonstrate here qualitatively (in images) and quantitatively (in terms of crater cone angles, depths, diameters and volume) laser ablation crater analysis in 3D for metal (aluminum) and rock (false gold ore). We show the effect of a Gaussian beam profile on the resulting crater geometry, as well as the first visual evidence of undercutting in the rock sample, most likely due to ejection of relatively large grains. The method holds promise for optimization of laser ablation setups especially for laser induced breakdown spectroscopy.

  3. Proton- and x-ray beams generated by ultra-fast CO2 lasers for medical applications

    Science.gov (United States)

    Pogorelsky, Igor; Polyanskiy, Mikhail; Yakimenko, Vitaly; Ben-Zvi, Ilan; Shkolnikov, Peter; Najmudin, Zulfikar; Palmer, Charlotte A. J.; Dover, Nicholas P.; Oliva, Piernicola; Carpinelli, Massimo

    2011-05-01

    Recent progress in using picosecond CO2 lasers for Thomson scattering and ion-acceleration experiments underlines their potentials for enabling secondary radiation- and particle- sources. These experiments capitalize on certain advantages of long-wavelength CO2 lasers, such as higher number of photons per energy unit, and favorable scaling of the electrons' ponderomotive energy and critical plasma density. The high-flux x-ray bursts produced by Thomson scattering of the CO2 laser off a counter-propagating electron beam enabled high-contrast, time-resolved imaging of biological objects in the picosecond time frame. In different experiments, the laser, focused on a hydrogen jet, generated monoenergetic proton beams via the radiation-pressure mechanism. The strong power-scaling of this regime promises realization of proton beams suitable for laser-driven proton cancer therapy after upgrading the CO2 laser to sub-PW peak power. This planned improvement includes optimizing the 10-μm ultra-short pulse generation, assuring higher amplification in the CO2 gas under combined isotopic- and power-broadening effects, and shortening the postamplification pulse to a few laser cycles (150-200 fs) via chirping and compression. These developments will move us closer to practical applications of ultra-fast CO2 lasers in medicine and other areas.

  4. Spatially resolved soft x-ray diagnostics in fusion energy research

    International Nuclear Information System (INIS)

    Mlynar, J.; Weinzettl, V.; Imrisek, M.; Loeffelmann, V.

    2013-01-01

    With construction of ITER, the fusion community has progressed into a new stage of research with increased focus on reactor technologies. Corresponding development of diagnostic systems for fusion is required, including research of novel diagnostic methods, validation of radiation hard detectors, and tests of sensors for real-time operation and control, which comprise development of tools for fast data analyses. In parallel, diagnostic systems on running fusion experiments substantially contribute to better understanding of reactor-relevant plasma physics, in particular of energy confinement, plasma stability and transport of impurities. In this respect, spatially resolved Soft X-ray (SXR) diagnostic systems present an interesting case study of development towards reactor-relevant systems. In magnetic confinement fusion research, spatial distribution of SXR radiation with spectral range typically 1 keV - 15 keV is mostly measured by a photosensitive single-row semiconductor elements in a pinhole camera shielded by a beryllium foil. The SXR intensity strongly depends on plasma density, temperature and effective charge, which carry a valuable information on the plasma core physics. Data from SXR diagnostic can be also used for the operation control, among others due to their sensitivity to heavy impurity concentration or to the position of the peak temperature. In order to reconstruct the spatial distribution of SXR plasma emission from the measured line integrated signals, several tomographic methods have been developed and validated. However, the semiconductor elements cannot survive in harsh conditions of future fusion reactors due to radiation damage, which calls for development of radiation hard SXR cameras. In this contribution, role of the SXR diagnostics will be presented in experience and future plans of the Czech tokamak COMPASS (IPP Prague) and the French tokamak TORE SUPRA (CEA Cadarache). In IPP Prague, data from SXR cameras recently contributed to

  5. Ultrafast cavitation induced by an X-ray laser in water drops

    Science.gov (United States)

    Stan, Claudiu; Willmott, Philip; Stone, Howard; Koglin, Jason; Liang, Mengning; Aquila, Andrew; Robinson, Joseph; Gumerlock, Karl; Blaj, Gabriel; Sierra, Raymond; Boutet, Sebastien; Guillet, Serge; Curtis, Robin; Vetter, Sharon; Loos, Henrik; Turner, James; Decker, Franz-Josef

    2016-11-01

    Cavitation in pure water is determined by an intrinsic heterogeneous cavitation mechanism, which prevents in general the experimental generation of large tensions (negative pressures) in bulk liquid water. We developed an ultrafast decompression technique, based on the reflection of shock waves generated by an X-ray laser inside liquid drops, to stretch liquids to large negative pressures in a few nanoseconds. Using this method, we observed cavitation in liquid water at pressures below -100 MPa. These large tensions exceed significantly those achieved previously, mainly due to the ultrafast decompression. The decompression induced by shock waves generated by an X-ray laser is rapid enough to continue to stretch the liquid phase after the heterogeneous cavitation occurs in water, despite the rapid growth of cavitation nanobubbles. We developed a nucleation-and-growth hydrodynamic cavitation model that explains our results and estimates the concentration of heterogeneous cavitation nuclei in water.

  6. High average power, highly brilliant laser-produced plasma source for soft X-ray spectroscopy.

    Science.gov (United States)

    Mantouvalou, Ioanna; Witte, Katharina; Grötzsch, Daniel; Neitzel, Michael; Günther, Sabrina; Baumann, Jonas; Jung, Robert; Stiel, Holger; Kanngiesser, Birgit; Sandner, Wolfgang

    2015-03-01

    In this work, a novel laser-produced plasma source is presented which delivers pulsed broadband soft X-radiation in the range between 100 and 1200 eV. The source was designed in view of long operating hours, high stability, and cost effectiveness. It relies on a rotating and translating metal target and achieves high stability through an on-line monitoring device using a four quadrant extreme ultraviolet diode in a pinhole camera arrangement. The source can be operated with three different laser pulse durations and various target materials and is equipped with two beamlines for simultaneous experiments. Characterization measurements are presented with special emphasis on the source position and emission stability of the source. As a first application, a near edge X-ray absorption fine structure measurement on a thin polyimide foil shows the potential of the source for soft X-ray spectroscopy.

  7. Undulator commissioning by characterization of radiation in x-ray free electron lasers

    Directory of Open Access Journals (Sweden)

    Takashi Tanaka

    2012-11-01

    Full Text Available In x-ray free electron lasers (XFELs where a long undulator composed of many segments is installed, there exist a number of error sources to reduce the FEL gain such as the trajectory error, K value discrepancy, and phase mismatch, which are related to the segmented-undulator structure. Undulator commissioning, which refers to the tuning and alignment processes to eliminate the possible error sources, is thus an important step toward realization of lasing. In the SPring-8 angstrom compact free electron laser (SACLA facility, the undulator commissioning has been carried out by means of characterization of x-ray radiation, i.e., measurements of the spatial and spectral profiles of monochromatized spontaneous undulator radiation as well as by probing the FEL intensity. The achieved tuning and alignment accuracies estimated from the statistics of actual measurements in SACLA show the effectiveness of this commissioning scheme.

  8. Difference structures from time-resolved small-angle and wide-angle x-ray scattering

    Science.gov (United States)

    Nepal, Prakash; Saldin, D. K.

    2018-05-01

    Time-resolved small-angle x-ray scattering/wide-angle x-ray scattering (SAXS/WAXS) is capable of recovering difference structures directly from difference SAXS/WAXS curves. It does so by means of the theory described here because the structural changes in pump-probe detection in a typical time-resolved experiment are generally small enough to be confined to a single residue or group in close proximity which is identified by a method akin to the difference Fourier method of time-resolved crystallography. If it is assumed, as is usual with time-resolved structures, that the moved atoms lie within the residue, the 100-fold reduction in the search space (assuming a typical protein has about 100 residues) allows the exaction of the structure by a simulated annealing algorithm with a huge reduction in computing time and leads to a greater resolution by varying the positions of atoms only within that residue. This reduction in the number of potential moved atoms allows us to identify the actual motions of the individual atoms. In the case of a crystal, time-resolved calculations are normally performed using the difference Fourier method, which is, of course, not directly applicable to SAXS/WAXS. The method developed in this paper may be thought of as a substitute for that method which allows SAXS/WAXS (and hence disordered molecules) to also be used for time-resolved structural work.

  9. Comparison of simulation to absolute X-ray emission of CH plasma created with the Nike laser

    Energy Technology Data Exchange (ETDEWEB)

    Busquet, M.; Feldman, U.; Klapisch, M. [ARTEP, Inc., Ellicott City, Maryland (contractor to NRL) (United States); Weaver, J.L.; Colombant, D.G.; Mostovych, A.N. [Naval Research Laboratory, Plasma Physics Division, Washington, DC (United States); Seely, J.F. [Naval Research Laboratory, Space Science Division, Washington, DC (United States); Holland, G. [SFA, Inc., Landover, Maryland (contractor to NRL) (United States)

    2006-06-15

    The Nike laser group at the Naval Research Laboratory has an ongoing effort to improve and benchmark the radiation hydrodynamic simulations used to develop pellet designs for inertial confinement fusion. A new post-processor, Virtual Spectro, has been added to the FAST code suite for detailed simulation of non-local thermodynamical equilibrium (non-LTE) spectra, including radiation transport effects and Stark line profile. This new combination enhances our ability to predict the absolute emission of soft X-rays. An absolutely calibrated transmission grating spectrometer and a high resolution grazing incidence spectrometer have been used to collect time integrated and time resolved spectra emitted by CH targets irradiated at laser intensities of about 10 TW/cm{sup 2}. Comparison between these observations and simulations using Virtual Spectro demonstrates excellent agreement (within factor of about 1.5) for the absolute emission. (authors)

  10. Comparison of simulation to absolute X-ray emission of CH plasma created with the Nike laser

    International Nuclear Information System (INIS)

    Busquet, M.; Feldman, U.; Klapisch, M.; Weaver, J.L.; Colombant, D.G.; Mostovych, A.N.; Seely, J.F.; Holland, G.

    2006-01-01

    The Nike laser group at the Naval Research Laboratory has an ongoing effort to improve and benchmark the radiation hydrodynamic simulations used to develop pellet designs for inertial confinement fusion. A new post-processor, Virtual Spectro, has been added to the FAST code suite for detailed simulation of non-local thermodynamical equilibrium (non-LTE) spectra, including radiation transport effects and Stark line profile. This new combination enhances our ability to predict the absolute emission of soft X-rays. An absolutely calibrated transmission grating spectrometer and a high resolution grazing incidence spectrometer have been used to collect time integrated and time resolved spectra emitted by CH targets irradiated at laser intensities of about 10 TW/cm 2 . Comparison between these observations and simulations using Virtual Spectro demonstrates excellent agreement (within factor of about 1.5) for the absolute emission. (authors)

  11. X-ray emission from plasmas created by smoothed KrF laser irradiation

    International Nuclear Information System (INIS)

    Aglitskiy, Y.; Lehecka, T.; Deniz, A.; Hardgrove, J.; Seely, J.; Brown, C.; Feldman, U.; Pawley, C.; Gerber, K.; Bodner, S.; Obenschain, S.; Lehmberg, R.; McLean, E.; Pronko, M.; Sethian, J.; Stamper, J.; Schmitt, A.; Sullivan, C.; Holland, G.; Laming, M.

    1996-01-01

    The x-ray emission from plasmas created by the Naval Research Laboratory Nike KrF laser [Phys. Plasmas 3, 2098 (1996) ] was characterized using imaging and spectroscopic instruments. The laser wavelength was 1/4 μm, and the beams were smoothed by induced spatial incoherence (ISI). The targets were thin foils of CH, aluminum, titanium, and cobalt and were irradiated by laser energies in the range 100 endash 1500 J. A multilayer mirror microscope operating at an energy of 95 eV recorded images of the plasma with a spatial resolution of 2 μm. The variation of the 95 eV emission across the 800 μm focal spot was 1.3% rms. Using a curved crystal imager operating in the 1 endash 2 keV x-ray region, the density, temperature, and opacity of aluminum plasmas were determined with a spatial resolution of 10 μm perpendicular to the target surface. The spectral line ratios indicated that the aluminum plasmas were relatively dense, cool, and optically thick near the target surface. The absolute radiation flux was determined at 95 eV and in x-ray bandpasses covering the 1 endash 8 keV region. The electron temperature inferred from the slope of the x-ray flux versus energy data in the 5 endash 8 keV region was 900 eV for an incident laser energy of 200 J and an intensity of ≅10 13 W/cm 2

  12. X-ray imaging of targets irradiated by the Nike KrF laser

    International Nuclear Information System (INIS)

    Brown, C.; Seely, J.; Feldman, U.; Obenschain, S.; Bodner, S.; Pawley, C.; Gerber, K.; Serlin, V.; Sethian, J.; Aglitskiy, Y.; Lehecka, T.; Holland, G.

    1997-01-01

    Foil targets irradiated by the Naval Research Laboratory Nike KrF laser were imaged in the x-ray region with two-dimensional spatial resolution in the 2 endash 10 μm range. The images revealed the smoothness of the emission from target and backlighter foils, the acceleration of the target foils, and the growth of Rayleigh endash Taylor instabilities that were seeded by patterns on the irradiated sides of CH foils

  13. Functional characterization of planar sensors with active edges using laser and X-ray beam scans

    International Nuclear Information System (INIS)

    Povoli, M.; Bagolini, A.; Boscardin, M.; Dalla Betta, G.-F.; Giacomini, G.; Hasi, J.; Oh, A.; Zorzi, N.

    2013-01-01

    We report on the functional characterization of planar sensors with active edges fabricated at Fondazione Bruno Kessler (FBK), Trento, Italy. The measurements here reported were performed by means of laser and X-ray beam scans mainly focusing on the signal efficiency of the edge region of the devices. Results are very encouraging and show very good sensitivity up to few microns away from the device physical edge

  14. Functional characterization of planar sensors with active edges using laser and X-ray beam scans

    Energy Technology Data Exchange (ETDEWEB)

    Povoli, M., E-mail: povoli@disi.unitn.it [Dipartimento di Ingegneria e Scienza dell' Informazione, Università di Trento, Via Sommarive, 14, I-38123 Povo di Trento (Italy); INFN, Sezione di Padova (Gruppo Collegato di Trento),Via Sommarive, 14, I-38123 Povo di Trento (Italy); Bagolini, A.; Boscardin, M. [Fondazione Bruno Kessler, Centro per i Materiali e i Microsistemi (FBK-CMM), Via Sommarive, 18, I-38123 Povo di Trento (Italy); Dalla Betta, G.-F. [Dipartimento di Ingegneria e Scienza dell' Informazione, Università di Trento, Via Sommarive, 14, I-38123 Povo di Trento (Italy); INFN, Sezione di Padova (Gruppo Collegato di Trento),Via Sommarive, 14, I-38123 Povo di Trento (Italy); Giacomini, G. [Fondazione Bruno Kessler, Centro per i Materiali e i Microsistemi (FBK-CMM), Via Sommarive, 18, I-38123 Povo di Trento (Italy); Hasi, J. [SLAC National Accelerator Laboratory, 2575 Sand Hill Road, Menlo Park, CA 94025-7015 (United States); Oh, A. [The University of Manchester, Oxford Road, Manchester M13 9PL (United Kingdom); Zorzi, N. [Fondazione Bruno Kessler, Centro per i Materiali e i Microsistemi (FBK-CMM), Via Sommarive, 18, I-38123 Povo di Trento (Italy)

    2013-08-01

    We report on the functional characterization of planar sensors with active edges fabricated at Fondazione Bruno Kessler (FBK), Trento, Italy. The measurements here reported were performed by means of laser and X-ray beam scans mainly focusing on the signal efficiency of the edge region of the devices. Results are very encouraging and show very good sensitivity up to few microns away from the device physical edge.

  15. Optimized K (alpha) x-ray flashes from femtosecond-laser-irradiated foils

    Czech Academy of Sciences Publication Activity Database

    Lu, W.; Nicoul, M.; Shymanovich, U.; Tarasevitch, A.; Zhou, P.; Sokolowski-Tinten, K.; von der Linde, D.; Mašek, Martin; Gibbon, P.; Teubner, U.

    2009-01-01

    Roč. 80, č. 2 (2009), 026404/1-026404/10 ISSN 1539-3755 R&D Projects: GA MŠk(CZ) LC528 Institutional research plan: CEZ:AV0Z10100523 Keywords : copper * electron density * high-speed optical techniques * plasma density * plasma production by laser * plasma simulation * plasma x-ray sources * titanium Subject RIV: BL - Plasma and Gas Discharge Physics Impact factor: 2.400, year: 2009

  16. Route to Soft X-ray Laser Pumped by Gas-Filled-Capillary Discharge

    Czech Academy of Sciences Publication Activity Database

    Koláček, Karel; Schmidt, Jiří; Prukner, Václav; Řípa, Milan; Frolov, Oleksandr; Štraus, Jaroslav; Vrba, Pavel

    2004-01-01

    Roč. 34, - (2004), s. 154-157 ISSN 1433-5581. [First Cairo Conference on Plasma Physics & Applications. Cairo, 11.10.2003-15.10.2003] R&D Projects: GA ČR(CZ) GA202/03/0711 Grant - others:GA MŠk1(CZ) LA 235 Keywords : fast capillary discharge * soft x-Ray laser Subject RIV: BL - Plasma and Gas Discharge Physics

  17. Femtosecond and Subfemtosecond X-Ray Pulses from a SASE Based Free-Electron Laser

    Energy Technology Data Exchange (ETDEWEB)

    Emma, P

    2004-03-10

    We propose a novel method to generate femtosecond and sub-femtosecond photon pulses in a free electron laser by selectively spoiling the transverse emittance of the electron beam. Its merits are simplicity and ease of implementation. When the system is applied to the Linac Coherent Light Source, it can provide x-ray pulses the order of 1 femtosecond in duration containing about 1010 transversely coherent photons.

  18. KMSF x-ray laser experiments. Task No. 2. Final report

    International Nuclear Information System (INIS)

    Charatis, G.

    1984-07-01

    This report summarizes work done at KMS Fusion, Inc. in support of the x-ray laser experimental program at Lawrence Livermore National Laboratory. It follows an earlier report of Task No. 1 of the subject purchase order. As in that report, most of the original data has been reviewed by the LLNL technical staff, with much of it transferred to LLNL for analysis. Consequently, this report does not include a detailed presentation of the data

  19. Modelling of a Nitrogen X-ray Laser pumped by Capillary Discharge

    Czech Academy of Sciences Publication Activity Database

    Vrba, Pavel; Vrbová, M.; Bobrova, N. A.; Sasorov, P. V.

    2005-01-01

    Roč. 3, č. 4 (2005), s. 564-580 ISSN 1644-3608 R&D Projects: GA MŠk(CZ) 1P04LA235 Institutional research plan: CEZ:AV0Z20430508 Keywords : MHD simulations * Z-pinch * Ion kinetics * Recombination Pumping * X-Ray laser Subject RIV: BL - Plasma and Gas Discharge Physics Impact factor: 0.524, year: 2005

  20. Analysis of the x-ray spectrum emitted by laser-produced plasma of dysprosium

    International Nuclear Information System (INIS)

    Marcus, Gilad; Louzon, Einat; Henis, Zohar; Maman, Shlomo; Mandelbaum, Pinchas

    2007-01-01

    A detailed analysis of the x-ray spectrum (5-10.2 A ring ) emitted by laser-produced plasma of dysprosium (Dy) is given using ab initio calculations with the HULLAC relativistic code and isoelectronic trends. Resonance 3d-4p, 3d-nf (n=4 to 7), 3p-4s, and 3p-4d transitions of Ni I-like Dy XXXIX and neighboring ion satellite transitions (from Dy XXXIV to Dy XL) are identified

  1. Coherence Properties of Individual Femtosecond Pulses of an X-ray Free-Electron Laser

    Energy Technology Data Exchange (ETDEWEB)

    Vartanyants, I.A.; /DESY /Moscow Phys. Eng. Inst.; Singer, A.; Mancuso, A.P.; Yefanov, O.M.; /DESY; Sakdinawat, A.; Liu, Y.; Bang, E.; /UC, Berkeley; Williams, G.J.; /SLAC; Cadenazzi, G.; Abbey, B.; /Melbourne U.; Sinn, H.; /European XFEL, Hamburg; Attwood, D.; /UC, Berkeley; Nugent, K.A.; /Melbourne U.; Weckert, E.; /DESY; Wang, T.; Zhu, D.; Wu, B.; Graves, C.; Scherz, A.; Turner, J.J.; Schlotter, W.F.; /SLAC /LERMA, Ivry /Zurich, ETH /LBL, Berkeley /ANL, APS /Argonne /SLAC /LLNL, Livermore /Latrobe U. /SLAC /SLAC /European XFEL, Hamburg /SLAC /Hamburg U.

    2012-06-06

    Measurements of the spatial and temporal coherence of single, femtosecond x-ray pulses generated by the first hard x-ray free-electron laser, the Linac Coherent Light Source, are presented. Single-shot measurements were performed at 780 eV x-ray photon energy using apertures containing double pinholes in 'diffract-and-destroy' mode. We determined a coherence length of 17 {micro}m in the vertical direction, which is approximately the size of the focused Linac Coherent Light Source beam in the same direction. The analysis of the diffraction patterns produced by the pinholes with the largest separation yields an estimate of the temporal coherence time of 0.55 fs. We find that the total degree of transverse coherence is 56% and that the x-ray pulses are adequately described by two transverse coherent modes in each direction. This leads us to the conclusion that 78% of the total power is contained in the dominant mode.

  2. Formation of x-ray Newton’s rings from nano-scale spallation shells of metals in laser ablation

    Directory of Open Access Journals (Sweden)

    Masaharu Nishikino

    2017-01-01

    Full Text Available The initial stages of the femtosecond (fs laser ablation process of gold, platinum, and tungsten were observed by single-shot soft x-ray imaging technique. The formation and evolution of soft x-ray Newton’s rings (NRs were found for the first time. The soft x-ray NRs are caused by the interference between the bulk ablated surface and nanometer-scale thin spallation layer; they originate from the metal surface at pump energy fluence of around 1 J/cm2 and work as a flying soft x-ray beam splitter.

  3. CMOS-sensors for energy-resolved X-ray imaging

    International Nuclear Information System (INIS)

    Doering, D.; Amar-Youcef, S.; Deveaux, M.; Linnik, B.; Müntz, C.; Stroth, Joachim; Baudot, J.; Dulinski, W.; Kachel, M.

    2016-01-01

    Due to their low noise, CMOS Monolithic Active Pixel Sensors are suited to sense X-rays with a few keV quantum energy, which is of interest for high resolution X-ray imaging. Moreover, the good energy resolution of the silicon sensors might be used to measure this quantum energy. Combining both features with the good spatial resolution of CMOS sensors opens the potential to build ''color sensitive' X-ray cameras. Taking such colored images is hampered by the need to operate the CMOS sensors in a single photon counting mode, which restricts the photon flux capability of the sensors. More importantly, the charge sharing between the pixels smears the potentially good energy resolution of the sensors. Based on our experience with CMOS sensors for charged particle tracking, we studied techniques to overcome the latter by means of an offline processing of the data obtained from a CMOS sensor prototype. We found that the energy resolution of the pixels can be recovered at the expense of reduced quantum efficiency. We will introduce the results of our study and discuss the feasibility of taking colored X-ray pictures with CMOS sensors

  4. Quantitative measurements with x-ray microscopes in laser-fusion experiments

    International Nuclear Information System (INIS)

    Marshall, F.J.; Su, Q.

    1995-01-01

    X-ray imaging of laser-fusion target implosions has been performed on the University of Rochester's OMEGA laser system by means of grazing-incidence optical imaging with Kirkpatrick--Baez (KB) microscopes. High spatial resolution imaging (∼5 μm) of hard x-ray emission (up to ∼7 keV) has been achieved. New grazing-incidence optics are currently being fabricated for the OMEGA Upgrade experimental laser-fusion facility. Projected performance indicates that resolution may be increased to ∼2 μm at the center of the field of view and sensitivity extended to ∼8 keV. Uses of KB microscopes on the OMEGA Upgrade will include hard x-ray imaging, grating-dispersed imaged spectroscopy, and framed imaging. A novel technique for monochromatic imaging with KB microscopes has also been demonstrated enabling images of target emission in a narrow energy band (10 to 20 eV) to be obtained

  5. Time Integrated Soft X-ray Imaging in High Intensity Laser Experiments (thesis)

    Energy Technology Data Exchange (ETDEWEB)

    Stafford, David [Univ. of California, Davis, CA (United States)

    2009-01-01

    2009 marks a significant achievement and the dawn of a new era in high intensity laser research with the final commissioning of all 192 beams at the National Ignition Facility (NIF). NIF is a department of energy (DOE) funded project more than 10 years in the making located at the Lawrence Livermore National Laboratory (LLNL). The following research was done as one of many preliminary experiments done to prepare for these historic events. The primary focus of the experimental campaign this paper addresses is to test and develop a thermal x-radiation source using a short pulse laser. This data is hoped to provide information about the thermal transport mechanisms important in the development of prediction models in High Energy Density (HED) science. One of several diagnostics fielded was a soft x-ray imager (SXRI) which is detailed in this paper. The SXRI will be used to measure the relative size of the heated region and also the relative level of specific x-ray emissions among several shot and target configurations. The laser system used was the Titan laser located in the Jupiter Laser Facility (JLF) at Lawrence Livermore National Laboratory (LLNL). Titan uses the JLF Janus Nd:glass laser west frontend system with a Optical Parametric Chirped Pulse Amplification (OPCPA) in place of the nanosecond oscillator. The system is capable of producing laser intensities of over a petawatt with several tens of joules delivered in the beam.

  6. Velocity-Resolved [Ne III] from X-Ray Irradiated Sz 102 Microjets

    Science.gov (United States)

    Liu, C.-F.; Shang, H.; Walter, F. M.; Herczeg, G. J.

    2014-03-01

    Neon emission lines are good indicators of high-excitation regions close to a young stellar system because of their high ionization potentials and large critical densities. We have discovered [Ne III] .3869 emission from the microjet of low-mass young star Sz 102. Spectroastrometric analysis of the two-dimensional [Ne III] spectral image obtained from the archival high-dispersion (R - 33,000) Very Large Telescope/UVES spectra suggests that the emission consists of two velocity components spatially separated by ~ 0.''3. The stronger redshifted component is centered at ~ +21 km s-1 with a line width of ~ 140 km s-1, and the weaker blueshifted component at ~ -90 km s-1 with a larger line width of ~ 190 km s-1. Both components have large line widths that extend across the systemic velocity, suggesting their origin from diverging streamlines of a wide-angle wind. Optical line ratio diagnostics indicate that Sz 102 drives a pair of hot (T . 2 ◊ 104 K) and ionized (ne . 2 ◊ 104 cm-3) jets. The blueshifted jet has on average ~ 50% higher temperature and electron density. We suggest that the jet is ionized by an embedded hard X-ray source close to the driving region. Freezing-in of the ionization state is consistent with the flow speed and the Ne2+ recombination timescales. We postulate that these X-rays originate from hard coronae or stellar flares; the hard (keV) X-ray photons ionize neon in the inner wind, while the soft X-rays are mostly absorbed by the accretion funnel. These postulates await validation from high-sensitivity X-ray and subarcsecond resolution optical observations.

  7. X-ray spectroscopy of a thin foil plasma produced by a short-pulse high-intensity laser

    International Nuclear Information System (INIS)

    Audebert, P.; Nagels, V.; Geindre, J.P.; Dorchies, F.; Peyrusse, O.; Gary, S.; Girard, F.; Shepherd, R.; Gauthier, J.C.; Chenais-Popovics, C.

    2003-01-01

    High density and temperature plasmas have been generated by irradiating thin foils of various elements with a high-energy subpicosecond laser pulse. The X-ray emission duration was studied by time-resolved X-ray spectroscopy. Frequency domain interferometry provided a measurement of the hydrodynamic expansion of the back of the foil as a function of time. The effect of longitudinal temperature gradients, i.e., gradients perpendicular to the surface, were decreased using very thin foil targets. Additionally, radial gradients effects, i.e., gradients parallel to the surface, were limited by using a 50 μm pinhole on target. The Al, Se and Sm spectra, recorded in the range 7.7-8 Angst. using a conical crystal spectrometer coupled to an 800 fs resolution streak camera, lasted a few picoseconds. Sm spectra showed no spectral features in this wavelength range, providing a spectrally homogeneous backlighter for future experiments. The main features of the experimental time-resolved spectra have been well reproduced with one-dimensional hydrodynamic simulations of the free expansion of a plasma heated at a given initial temperature obtained from the expansion velocity of the rear critical surface of the plasma

  8. A laser driven pulsed X-ray backscatter technique for enhanced penetrative imaging.

    Science.gov (United States)

    Deas, R M; Wilson, L A; Rusby, D; Alejo, A; Allott, R; Black, P P; Black, S E; Borghesi, M; Brenner, C M; Bryant, J; Clarke, R J; Collier, J C; Edwards, B; Foster, P; Greenhalgh, J; Hernandez-Gomez, C; Kar, S; Lockley, D; Moss, R M; Najmudin, Z; Pattathil, R; Symes, D; Whittle, M D; Wood, J C; McKenna, P; Neely, D

    2015-01-01

    X-ray backscatter imaging can be used for a wide range of imaging applications, in particular for industrial inspection and portal security. Currently, the application of this imaging technique to the detection of landmines is limited due to the surrounding sand or soil strongly attenuating the 10s to 100s of keV X-rays required for backscatter imaging. Here, we introduce a new approach involving a 140 MeV short-pulse (< 100 fs) electron beam generated by laser wakefield acceleration to probe the sample, which produces Bremsstrahlung X-rays within the sample enabling greater depths to be imaged. A variety of detector and scintillator configurations are examined, with the best time response seen from an absorptive coated BaF2 scintillator with a bandpass filter to remove the slow scintillation emission components. An X-ray backscatter image of an array of different density and atomic number items is demonstrated. The use of a compact laser wakefield accelerator to generate the electron source, combined with the rapid development of more compact, efficient and higher repetition rate high power laser systems will make this system feasible for applications in the field. Content includes material subject to Dstl (c) Crown copyright (2014). Licensed under the terms of the Open Government Licence except where otherwise stated. To view this licence, visit http://www.nationalarchives.gov.uk/doc/open-government-licence/version/3 or write to the Information Policy Team, The National Archives, Kew, London TW9 4DU, or email: psi@ nationalarchives.gsi.gov.uk.

  9. Performance of soft x-ray laser pumped by capillary discharge

    International Nuclear Information System (INIS)

    Sakai, Yusuke; Kakuya, Yuji; Xiao, Yifan

    2005-01-01

    We report the output characteristics of capillary discharge single-pass 46.9 nm Ne-like Ar soft-X-ray laser generated by a capillary z-pinch discharge. The coherence properties of the laser have shown to be improved with the increase of the length of laser amplifier from 20 up to 35 cm. The high degree of the spatial coherence of the laser beam produced by 35 cm long capillary is demonstrated by the results obtained in a classical Young's double-slit experiments. We found that the coherence length of the laser is 50 μm. For the 20 cm-long capillary, the diameter of a laser beam is in a range from 3.2 to 4.0 mm, which is corresponding to a range of divergence from 2.2 to 2.8 mrad. Finally, we introduce two spikes on X-ray diode (XRD) signal observed in a single shot. (author)

  10. Time-resolved X-ray scattering by electronic wave packets: analytic solutions to the hydrogen atom

    DEFF Research Database (Denmark)

    Simmermacher, Mats; Henriksen, Niels Engholm; Møller, Klaus Braagaard

    2017-01-01

    Modern pulsed X-ray sources permit time-dependent measurements of dynamical changes in atoms and molecules via non-resonant scattering. The planning, analysis, and interpretation of such experiments, however, require a firm and elaborated theoretical framework. This paper provides a detailed...... description of time-resolved X-ray scattering by non-stationary electronic wave packets in atomic systems. A consistent application of the Waller-Hartree approximation is discussed and different contributions to the total differential scattering signal are identified and interpreted. Moreover......, it is demonstrated how the scattering signal of wave packets in the hydrogen atom can be expressed analytically. This permits simulations without numerical integration and establishes a benchmark for both efficiency and accuracy. Based on that, scattering patterns of an exemplary wave packet in the hydrogen atom...

  11. Self-consistent one-dimensional modelling of x-ray laser plasmas

    International Nuclear Information System (INIS)

    Wan, A.S.; Walling, R.S.; Scott, H.A.; Mayle, R.W.; Osterheld, A.L.

    1992-01-01

    This paper presents the simulation of a planar, one-dimensional expanding Ge x-ray laser plasma using a new code which combines hydrodynamics, laser absorption, and detailed level population calculations within the same simulation. Previously, these simulations were performed in separate steps. We will present the effect of line transfer on gains and excited level populations and compare the line transfer result with simulations using escape probabilities. We will also discuss the impact of different atomic models on the accuracy of our simulation

  12. Phase-matched generation of coherent soft and hard X-rays using IR lasers

    Science.gov (United States)

    Popmintchev, Tenio V.; Chen, Ming-Chang; Bahabad, Alon; Murnane, Margaret M.; Kapteyn, Henry C.

    2013-06-11

    Phase-matched high-order harmonic generation of soft and hard X-rays is accomplished using infrared driving lasers in a high-pressure non-linear medium. The pressure of the non-linear medium is increased to multi-atmospheres and a mid-IR (or higher) laser device provides the driving pulse. Based on this scaling, also a general method for global optimization of the flux of phase-matched high-order harmonic generation at a desired wavelength is designed.

  13. X-ray laser studies using plasmas created by optical field ionization

    International Nuclear Information System (INIS)

    Krushelnick, K.M.; Tighe, W.; Suckewer, S.

    1995-01-01

    X-ray laser experiments involving the creation of fast recombining plasmas by optical field ionization of preformed targets were conducted. A nonlinear increase in the intensity of the 13.5nm Lyman-α line in Li III with the length of the target plasma was observed but only for distances less than the laser confocal parameter and for low plasma electron temperatures. Multiphoton pumping of resonant atomic transitions was also examined and the process of multiphoton ionization of FIII was found to be more probable than multiphoton excitation

  14. Pulse repetition frequency effects in a high average power x-ray preionized excimer laser

    International Nuclear Information System (INIS)

    Fontaine, B.; Forestier, B.; Delaporte, P.; Canarelli, P.

    1989-01-01

    Experimental study of waves damping in a high repetition rate excimer laser is undertaken. Excitation of laser active medium in a subsonic loop is achieved by means of a classical discharge, through transfer capacitors. The discharge stability is controlled by a wire ion plasma (w.i.p.) X-rays gun. The strong acoustic waves induced by the active medium excitation may lead to a decrease, at high PRF, of the energy per pulse. First results of the influence of a damping of induced density perturbations between two successive pulses are presented

  15. Monte Carlo simulation on hard X-ray dose produced in interaction between high intensity laser and solid target

    International Nuclear Information System (INIS)

    Yang Bo; Qiu Rui; Li Junli; Zhang Hui

    2014-01-01

    The X-ray dose produced in the interaction between high intensity laser and solid target was studied by simulation using Monte Carlo code. Compared with experimental results, the calculation model was verified. The calculation model was used to study the effect on X-ray dose with different electron temperatures, target materials (including Au, Cu and PE) and thicknesses. The results indicate that the X-ray dose is mainly determined by the electron temperature, and will be affected by the target parameters. X-ray dose of Au is about 1.2 times that of Cu, and is about 5 times that of PE (polyethylene). In addition, compared with other target thickness, when target thickness is the mean range of electron in the target, X-ray dose is relatively large. These results will provide references on evaluating the ionizing radiation dose for laser devices. (authors)

  16. Electron density measurement of a colliding plasma using soft x-ray laser interferometry

    International Nuclear Information System (INIS)

    Wan, A.S.; Back, C.A.; Barbee, T.W.Jr.; Cauble, R.; Celliers, P.; DaSilva, L.B.; Glenzer, S.; Moreno, J.C.; Rambo, P.W.; Stone, G.F.; Trebes, J.E.; Weber, F.

    1996-05-01

    The understanding of the collision and subsequent interaction of counter-streaming high-density plasmas is important for the design of indirectly-driven inertial confinement fusion (ICF) hohlraums. We have employed a soft x-ray Mach-Zehnder interferometer, using a Ne- like Y x-ray laser at 155 angstrom as the probe source, to study interpenetration and stagnation of two colliding plasmas. We observed a peaked density profile at the symmetry axis with a wide stagnation region with width of order 100 μm. We compare the measured density profile with density profiles calculated by the radiation hydrodynamic code LASNEX and a multi-specie fluid code which allows for interpenetration. The measured density profile falls in between the calculated profiles using collisionless and fluid approximations. By using different target materials and irradiation configurations, we can vary the collisionality of the plasma. We hope to use the soft x-ray laser interferometry as a mechanism to validate and benchmark our numerical codes used for the design and analysis of high-energy- density physics experiments

  17. Radiography in the X-ray region of a laser implosed microball

    International Nuclear Information System (INIS)

    Launspach, J.; Bayer, C.; Billon, D.; Decroisette, M.; Juraszek, D.; Meynial, D.

    1981-05-01

    The OCTAL laser of the Limeil CEA Research Center was used to realize the implosion of small targets containing a mixture of DT and to produce thermonuclear fusion reactions. The experimental device in which the experiments were carried out is called Camelia. Its main component is a vacuum chamber upon which the following elements are fixed: - devices for adjusting the focussing lenses; - a device for positioning targets; - extensive diagnostic means enabling the maximum amount of information to be obtained from each shot. These experiments were performed in order to study laser implosion mechanisms and to measure the density and temperature characteristics that can be reached in this way. The X-ray radiography device is relatively simple. It consists of an X-ray source, the target to be analyzed, one or two stenopies and a detector which is either a simple film (Kodak Kodirex) for diagnostics without temporal resolution or a scanning camera with a slit when temporal resolution is required. The device can be used: - without an x-ray source for emission diagnostics with spatio-temporal resolution, - to study the pre-heating of targets by radiography of the dust at the beginning of the implosion, - for diagnostics of the plasma core by radiography of dust after the implosion [fr

  18. Carbon Condensation during High Explosive Detonation with Time Resolved Small Angle X-ray Scattering

    Science.gov (United States)

    Hammons, Joshua; Bagge-Hansen, Michael; Nielsen, Michael; Lauderbach, Lisa; Hodgin, Ralph; Bastea, Sorin; Fried, Larry; May, Chadd; Sinclair, Nicholas; Jensen, Brian; Gustavsen, Rick; Dattelbaum, Dana; Watkins, Erik; Firestone, Millicent; Ilavsky, Jan; van Buuren, Tony; Willey, Trevor; Lawrence Livermore National Lab Collaboration; Los Alamos National Laboratory Collaboration; Washington State University/Advanced Photon Source Team

    Carbon condensation during high-energy detonations occurs under extreme conditions and on very short time scales. Understanding and manipulating soot formation, particularly detonation nanodiamond, has attracted the attention of military, academic and industrial research. An in-situ characterization of these nanoscale phases, during detonation, is highly sought after and presents a formidable challenge even with today's instruments. Using the high flux available with synchrotron X-rays, pink beam small angle X-ray scattering is able to observe the carbon phases during detonation. This experimental approach, though powerful, requires careful consideration and support from other techniques, such as post-mortem TEM, EELS and USAXS. We present a comparative survey of carbon condensation from different CHNO high explosives. This work was performed under the auspices of the US DOE by LLNL under Contract DE-AC52-07NA27344.

  19. Strain analysis of trabecular bone using time-resolved X-ray microtomography

    Czech Academy of Sciences Publication Activity Database

    Jiroušek, Ondřej; Zlámal, Petr; Kytýř, Daniel; Kroupa, M.

    2011-01-01

    Roč. 633, Suppl. 1 (2011), s. 148-151 ISSN 0168-9002. [International Workshop on Radiation Imaging Detectors /11./. Praha, 28.06.2009-02.07.2009] R&D Projects: GA ČR(CZ) GP103/07/P483 Institutional research plan: CEZ:AV0Z20710524 Keywords : trabecular bone * X-ray microtomography * strain analysis * intrinsic material properties Subject RIV: JB - Sensors, Measurment, Regulation Impact factor: 1.207, year: 2011

  20. 3-D Cellular Ultrastructure Can Be Resolved by X-ray Microscopy | Center for Cancer Research

    Science.gov (United States)

    X-ray microscopy (XRM) is more rapid than cryoelectron tomography or super-resolution fluorescence microscopy and could fill an important gap in current technologies used to investigate in situ three-dimensional structure of cells. New XRM methods developed by first author Gerd Schneider, Ph.D., working with James McNally. Ph.D., and a team of colleagues, is capable of revealing full cellular ultrastructure without requiring fixation, staining, or sectioning.

  1. LabVIEW-based X-ray detection system for laser compton scattering experiment

    International Nuclear Information System (INIS)

    Luo Wen; Xu Wang; Pan Qiangyan

    2010-01-01

    A LabVIEW-based X-ray detection system has been developed for laser-Compton scattering (LCS) experiment at the 100 MeV Linac of the Shanghai Institute of Applied Physics (SINAP). It mainly consists of a Si (Li) detector, readout electronics and a LabVIEW-based Data Acquisition (DAQ), and possesses the functions of signal spectrum displaying, acquisition control and simple online data analysis and so on. The performance test shows that energy and time resolutions of the system are 184 eV at 5.9 keV and ≤ 1% respectively and system instability is found to be 0.3‰ within a week. As a result, this X-ray detection system has low-cost and high-performance features and can meet the requirements of LCS experiment. (authors)

  2. Simulation Studies of the X-Ray Free-Electron Laser Oscillator

    International Nuclear Information System (INIS)

    Lindberg, R.R.; Shyd'ko, Y.; Kim, K.-J; Fawley, W.M.

    2009-01-01

    Simulations of the x-ray free-electron laser (FEL) oscillator are presented that include transverse effects and realistic Bragg crystal properties with the two-dimensional code GINGER. In the present cases considered the radiation divergence is much narrower than the crystal acceptance, and the numerical algorithm can be simplified by ignoring the finite angular bandwidth of the crystal. In this regime GINGER shows that the saturated x-ray pulses have 109 photons and are nearly Fourier-limited with peak powers in excess of 1 MW. Wealso include preliminary results for a four-mirror cavity that can be tuned in wavelength over a few percent, with future plans to incorporate the full transverse response of the Bragg crystals into GINGER to more accurately model this tunable source.

  3. Assessing the quantum physics impacts on future x-ray free-electron lasers

    Energy Technology Data Exchange (ETDEWEB)

    Schmitt, Mark J. [Los Alamos National Lab. (LANL), Los Alamos, NM (United States); Anisimov, Petr Mikhaylovich [Los Alamos National Lab. (LANL), Los Alamos, NM (United States)

    2017-10-06

    A new quantum mechanical theory of x-ray free electron lasers (XFELs) has been successfully developed that has placed LANL at the forefront of the understanding of quantum effects in XFELs. Our quantum theory describes the interaction of relativistic electrons with x-ray radiation in the periodic magnetic field of an undulator using the same mathematical formalism as classical XFEL theory. This places classical and quantum treatments on the same footing and allows for a continuous transition from one regime to the other eliminating the disparate analytical approaches previously used. Moreover, Dr. Anisimov, the architect of this new theory, is now considered a resource in the international FEL community for assessing quantum effects in XFELs.

  4. Study of laser-imploded core plasmas with an advanced Kirkpatrick endash Baez x-ray microscope

    International Nuclear Information System (INIS)

    Kodama, R.; Shiraga, H.; Miyanaga, M.; Matsushita, T.; Nakai, M.; Azechi, H.; Mima, K.; Kato, Y.

    1997-01-01

    We developed an advanced Kirkpatrick endash Baez (AKB) x-ray microscope which consisted of two hyperbolic mirrors and two elliptic mirrors. The spatial resolution of approx-lt 3 μm was realized over ∼1 mm diam. This AKB microscope was used for x-ray imaging in laser fusion experiments. Laser absorption nonuniformity with a large wave number on a spherical solid target or a plane slab target was estimated by measurements of x-ray emission from the target surface with the microscope. The x-ray images of the imploded core plasmas were also obtained with the AKB microscope, changing the laser focus condition and the laser energy balance. copyright 1997 American Institute of Physics

  5. Development of a compact laser-produced plasma soft X-ray source for radiobiology experiments

    Energy Technology Data Exchange (ETDEWEB)

    Adjei, Daniel, E-mail: nana.adjeidan@gmail.com [Institute of Optoelectronics, Military University of Technology, 2, Kaliskiego Str., 00-908 Warsaw (Poland); Radiation Protection Institute, Ghana Atomic Energy Commission, P.O. Box LG 80, Legon, Accra (Ghana); Ayele, Mesfin Getachew; Wachulak, Przemyslaw; Bartnik, Andrzej; Wegrzynski, Łukasz; Fiedorowicz, Henryk [Institute of Optoelectronics, Military University of Technology, 2, Kaliskiego Str., 00-908 Warsaw (Poland); Vyšín, Luděk [Institute of Physics, Czech Academy of Sciences, Na Slovance 2, 182 21 Prague 8 (Czech Republic); Faculty of Nuclear Sciences and Engineering Physics, Czech Technical University in Prague, Břehová 7, 115 19 Prague 1 (Czech Republic); Wiechec, Anna; Lekki, Janusz; Kwiatek, Wojciech M. [Institute of Nuclear Physics, Polish Academy of Sciences, 152, Radzikowskiego Str., 31-342 Cracow (Poland); Pina, Ladislav [Faculty of Nuclear Sciences and Engineering Physics, Czech Technical University in Prague, Břehová 7, 115 19 Prague 1 (Czech Republic); Davídková, Marie [Institute of Nuclear Physics, Czech Academy of Sciences, Řež (Czech Republic); Juha, Libor [Institute of Physics, Czech Academy of Sciences, Na Slovance 2, 182 21 Prague 8 (Czech Republic)

    2015-12-01

    A desk-top laser-produced plasma (LPP) source of soft X-rays (SXR) has been developed for radiobiology research. The source is based on a double-stream gas puff target, irradiated with the focused beam of a commercial Nd:YAG laser. The source has been optimized to get a maximum photon emission from LPP in the X-ray “water window” spectral wavelength range from 2.3 nm (i.e., an absorption edge of oxygen) to 4.4 nm (i.e., an absorption edge of carbon) (280–540 eV in photon energy units) by using argon gas-puff target and spectral filtering by free-standing thin foils. The present source delivers nanosecond pulses of soft X-rays at a fluence of about 4.2 × 10{sup 3} photons/μm{sup 2}/pulse on a sample placed inside the vacuum chamber. In this paper, the source design, radiation output characterization measurements and initial irradiation experiments are described. The source can be useful in addressing observations related to biomolecular, cellular and organisms’ sensitivity to pulsed radiation in the “water window”, where carbon atoms absorb X-rays more strongly than the oxygen, mostly present in water. The combination of the SXR source and the radiobiology irradiation layout, reported in this article, make possible a systematic investigation of relationships between direct and indirect action of ionizing radiation, an increase of a local dose in carbon-rich compartments of the cell (e.g., lipid membranes), an experimental estimation of a particular role of the Auger effect (in particular in carbon atoms) in the damage to biological systems, and the study of ionization/excitation-density (LET – Linear Energy Transfer) and dose-rate effects in radiobiology.

  6. Laser-pump/X-ray-probe experiments with electrons ejected from a Cu(111) target: space-charge acceleration.

    Science.gov (United States)

    Schiwietz, G; Kühn, D; Föhlisch, A; Holldack, K; Kachel, T; Pontius, N

    2016-09-01

    A comprehensive investigation of the emission characteristics for electrons induced by X-rays of a few hundred eV at grazing-incidence angles on an atomically clean Cu(111) sample during laser excitation is presented. Electron energy spectra due to intense infrared laser irradiation are investigated at the BESSY II slicing facility. Furthermore, the influence of the corresponding high degree of target excitation (high peak current of photoemission) on the properties of Auger and photoelectrons liberated by a probe X-ray beam is investigated in time-resolved pump and probe measurements. Strong electron energy shifts have been found and assigned to space-charge acceleration. The variation of the shift with laser power and electron energy is investigated and discussed on the basis of experimental as well as new theoretical results.

  7. Spatial coherence properties of a compact and ultrafast laser-produced plasma keV x-ray source

    International Nuclear Information System (INIS)

    Boschetto, D.; Mourou, G.; Rousse, A.; Mordovanakis, A.; Hou, Bixue; Nees, J.; Kumah, D.; Clarke, R.

    2007-01-01

    The authors use Fresnel diffraction from knife-edges to demonstrate the spatial coherence of a tabletop ultrafast x-ray source produced by laser-plasma interaction. Spatial coherence is achieved in the far field by producing micrometer-scale x-ray spot dimensions. The results show an x-ray source size of 6 μm that leads to a transversal coherence length of 20 μm at a distance of 60 cm from the source. Moreover, they show that the source size is limited by the spatial spread of the absorbed laser energy

  8. The application of photoconductive detectors to the measurement of x-ray production in laser produced plasmas

    International Nuclear Information System (INIS)

    Kania, D.R.; Bell, P.; Trebes, J.

    1987-08-01

    Photoconductive detectors (PCDs) offer an attractive alternative for the measurement of pulsed x-rays from laser produced plasmas. These devices are fast (FWHM ∼100 ps), sensitive and simple to use. We have used InP, GaAs, and Type IIa diamond as PCDs to measure x-rays emission from 100 eV to 100 keV. Specifically, we have used these detectors to measure total radiation yields, corona temperatures, and hot electron generated x-rays from laser produced plasmas. 5 refs., 4 figs

  9. Note: Diagnosing femtosecond laser-solid interactions with monochromatic Kα imager and x-ray pinhole camera

    International Nuclear Information System (INIS)

    Lin, X. X.; Li, Y. T.; Liu, F.; Du, F.; Wang, S. J.; Chen, L. M.; Zhang, L.; Zheng, Y.; Liu, X.; Liu, X. L.; Wang, Z. H.; Ma, J. L.; Wei, Z. Y.; Liu, B. C.; Zhang, J.

    2011-01-01

    An x-ray pinhole camera and a monochromatic K α imager are used to measure the interactions of intense femtosecond laser pulses with Cu foil targets. The two diagnostics give different features in the spot size and the laser energy scaling, which are resulted from different physical processes. Under our experimental conditons, the K α emission is mainly excited by the fast electrons transporting inside the cold bulk target. In contrast, the x-ray pinhole signals are dominated by the broadband thermal x-ray emission from the hot plasma at the front target surface.

  10. Temporal feature of X-ray laser plasma observed from 3ω0/2, 2ω0 harmonic emission

    International Nuclear Information System (INIS)

    Li Wenhong; Mei Qiyong; Zhao Xuewei; Chen Yuting; Chunyu Shutai

    1995-01-01

    Temporal feature of X-ray laser plasma density was observed from 3ω 0 /2, 2ω 0 harmonic emission in the experiments. The temporal feature of 3ω 0 /2 harmonic emission of the germanium film is much different from that of the slab germanium target. The production of x-ray laser is closely related to 3ω 0 /2 harmonic emission in the slab germanium targets

  11. Ultrashort X-ray pulse science

    Energy Technology Data Exchange (ETDEWEB)

    Chin, Alan Hap [Univ. of California, Berkeley, CA (US). Dept. of Physics; Lawrence Berkeley National Lab. (LBNL), Berkeley, CA (United States)

    1998-05-01

    A variety of phenomena involves atomic motion on the femtosecond time-scale. These phenomena have been studied using ultrashort optical pulses, which indirectly probe atomic positions through changes in optical properties. Because x-rays can more directly probe atomic positions, ultrashort x-ray pulses are better suited for the study of ultrafast structural dynamics. One approach towards generating ultrashort x-ray pulses is by 90° Thomson scattering between terawatt laser pulses and relativistic electrons. Using this technique, the author generated ~ 300 fs, 30 keV (0.4 Å) x-ray pulses. These x-ray pulses are absolutely synchronized with ultrashort laser pulses, allowing femtosecond optical pump/x-ray probe experiments to be performed. Using the right-angle Thomson scattering x-ray source, the author performed time-resolved x-ray diffraction studies of laser-perturbated InSb. These experiments revealed a delayed onset of lattice expansion. This delay is due to the energy relaxation from a dense electron-hole plasma to the lattice. The dense electron-hole plasma first undergoes Auger recombination, which reduces the carrier concentration while maintaining energy content. Longitudinal-optic (LO) phonon emission then couples energy to the lattice. LO phonon decay into acoustic phonons, and acoustic phonon propagation then causes the growth of a thermally expanded layer. Source characterization is instrumental in utilizing ultrashort x-ray pulses in time-resolved x-ray spectroscopies. By measurement of the electron beam diameter at the generation point, the pulse duration of the Thomson scattered x-rays is determined. Analysis of the Thomson scattered x-ray beam properties also provides a novel means of electron bunch characterization. Although the pulse duration is inferred for the Thomson scattering x-ray source, direct measurement is required for other x-ray pulse sources. A method based on the laser-assisted photoelectric effect (LAPE) has been demonstrated as a

  12. Ultrashort X-ray pulse science

    International Nuclear Information System (INIS)

    Chin, A.H.; Lawrence Berkeley National Lab., CA

    1998-01-01

    A variety of phenomena involves atomic motion on the femtosecond time-scale. These phenomena have been studied using ultrashort optical pulses, which indirectly probe atomic positions through changes in optical properties. Because x-rays can more directly probe atomic positions, ultrashort x-ray pulses are better suited for the study of ultrafast structural dynamics. One approach towards generating ultrashort x-ray pulses is by 90 o Thomson scattering between terawatt laser pulses and relativistic electrons. Using this technique, the author generated ∼ 300 fs, 30 keV (0.4 (angstrom)) x-ray pulses. These x-ray pulses are absolutely synchronized with ultrashort laser pulses, allowing femtosecond optical pump/x-ray probe experiments to be performed. Using the right-angle Thomson scattering x-ray source, the author performed time-resolved x-ray diffraction studies of laser-perturbated InSb. These experiments revealed a delayed onset of lattice expansion. This delay is due to the energy relaxation from a dense electron-hole plasma to the lattice. The dense electron-hole plasma first undergoes Auger recombination, which reduces the carrier concentration while maintaining energy content. Longitudinal-optic (LO) phonon emission then couples energy to the lattice. LO phonon decay into acoustic phonons, and acoustic phonon propagation then causes the growth of a thermally expanded layer. Source characterization is instrumental in utilizing ultrashort x-ray pulses in time-resolved x-ray spectroscopies. By measurement of the electron beam diameter at the generation point, the pulse duration of the Thomson scattered x-rays is determined. Analysis of the Thomson scattered x-ray beam properties also provides a novel means of electron bunch characterization. Although the pulse duration is inferred for the Thomson scattering x-ray source, direct measurement is required for other x-ray pulse sources. A method based on the laser-assisted photoelectric effect (LAPE) has been

  13. PROCEEDING OF THE SEEDED X-RAY FREE ELECTRON LASER WORKSHOP.

    Energy Technology Data Exchange (ETDEWEB)

    WANG,X.J.; MURPHY,J.B.; YU,L.H.; FAATZ,B.; HUANG,Z.; REICHE,S.; ZOLOTOREV,M.

    2002-12-13

    The underlying theory of a high gain free electron laser (FEL) has existed for two decades [1-2], but it is only in the last few years that these novel radiation sources have been realized experimentally. Several high gain FELs have successfully reached saturation in the infrared, visible and the VUV portion of the spectrum: the High Gain Harmonic Generation (HGHG) free electron lasers [3] at BNL and the Self Amplified Spontaneous Emission (SASE) FELs at LEUTL, VISA and TTF [4-6]. The outstanding challenges for future FELs are to extend high gain FELs to the X-ray regime, improve the longitudinal coherence of the radiation using seeded FEL schemes and generate ultrashort pulses (<100 fs). The National Synchrotron Light Source (NSLS) of the Brookhaven National Laboratory (BNL) sponsored a Seeded X-ray Free Electron Laser Workshop on December 13-14, 2002 to explore these challenging issues. Representatives from BNL, DESY, LBNL, SLAC and UCLA made presentations on the novel schemes under consideration at their laboratories. Workshop participants had a lively discussion on the feasibility, performance and R&D issues associated with the seeded XFEL schemes. An improvement of the electron beam quality will certainly be necessary to drive the XFEL. Self-seeding SASE, cascaded HGHG, and SASE pulse compression FELs show the most promise for producing short pulse X-rays. Of these, only the self-seeded and HGHG schemes generate longitudinally coherent radiation. While the pulse length in the self-seeded scheme is determined by the electron bunch length ({approx}100 fs), the pulse length in the HGHG scheme is determined by the short pulse seed laser, and so can be much shorter ({approx} 20 fs).

  14. Optimum discharge current waveforms for pumping Ne-like Ar soft X-ray laser

    International Nuclear Information System (INIS)

    Zhao Yongpeng; Jiang Shan; Xie Yao; Teng Shupeng; Wang Qi

    2011-01-01

    In order to enhance intensity of Ne-like Ar 46.9 nm soft X-ray laser pumped by capillary discharge, influences of main current waveform on Z-pinch process,time of lasing onset and laser intensity were studied. Rise-time of main current waveform was changed by varying conducting inductance of main switch. Experimental results with different rise-times show that amplitude of laser spike decreases with increasing rise-time,and time of lasing onset increases with increasing rise-time. In addition, influences of average current changing rate on laser intensity were studied. When inner diameter of capillary is 3 mm and initial pressure is 30 Pa, optimum average current changing rate is about 7.0 x 10 11 A/s. (authors)

  15. Spatially Resolved Hard X-ray Emission in the Central 5 kpc of the Galaxy Merger NGC 6240

    Science.gov (United States)

    Wang, Junfeng; Nardini, E.; Fabbiano, G.; Karovska, M.; Elvis, M.; Pellegrini, S.; Max, C. E.; Risaliti, G.; U, V.; Zezas, A.

    2013-04-01

    We have obtained a deep, sub-arcsecond resolution X-ray image of the nuclear region of the luminous galaxy merger NGC 6240 with Chandra, which resolves the X-ray emission from the pair of active nuclei and the diffuse hot gas in great detail. We detect extended hard X-ray emission from 70 million K hot gas over a spatial scale of 5 kpc, indicating the presence of fast shocks with velocity of 2200 km/s. For the first time we obtain spatial distribution of this highly ionized gas emitting FeXXV and find that it shows a remarkable correspondence to the large scale morphology of H_2(1-0) S(1) line emission and Hα filaments. Propagation of fast shocks originated in the starburst driven wind into the ambient dense gas can account for this morphological correspondence. Both the energetics and the iron mass in the hot gas are consistent with the expected injection from the supernovae explosion during the starburst that is commensurate with its high star formation rate.

  16. Experimental studies of x-ray laser spectral profiles: Observation of gain narrowing and saturation behavior

    International Nuclear Information System (INIS)

    Koch, J.A.; MacGowan, B.J.; Da Silva, L.B.; Matthews, D.L.; Mrowka, S.; Underwood, J.H.; Batson, P.J.

    1992-01-01

    We discuss our recent measurements of the spectral width of the 206.38 Angstrom x-ray laser transition in Ne-like Se. These measurements used a high-resolution grating spectrometer and were performed over a wide range of laser amplifier lengths. The data have enabled us to extrapolate the intrinsic line width and to observe the effects of gain-narrowing and saturation on the line profile. We find an intrinsic width which is 1.4 times the Doppler width, we observe gain-narrowing in intermediate length amplifiers, and we observe no re-broadening in long, saturated amplifiers. These results suggest that collisional line-broadening has a significant effect on the line profile and saturation behavior of this laser. We discuss modeling we have performed in order to simulate the experimental data, and we discuss future experimental and theoretical efforts we believe are necessary in order to understand line broadening and line transfer issues in x-ray laser plasmas

  17. A Novel Spectrometer for Measuring Laser-Produced Plasma X-Ray in Inertial Confinement Fusion

    Directory of Open Access Journals (Sweden)

    Zhu Gang

    2012-01-01

    Full Text Available In the experimental investigations of inertial confinement fusion, the laser-produced high-temperature plasma contains very abundant information, such as the electron temperature and density, ionization. In order to diagnose laser-plasma distribution in space and evolution in time, an elliptical curved crystal spectrometer has been developed and applied to diagnose X-ray of laser-produced plasma in 0.2~2.46 nm region. According to the theory of Bragg diffraction, four kinds of crystal including LiF, PET, MiCa, and KAP were chosen as dispersive elements. The distance of crystal lattice varies from 0.4 to 2.6 nm. Bragg angle is in the range of 30°~67.5°, and the spectral detection angle is in 55.4°~134°. The curved crystal spectrometer mainly consists of elliptical curved crystal analyzer, vacuum configuration, aligning device, spectral detectors and three-dimensional microadjustment devices. The spectrographic experiment was carried out on the XG-2 laser facility. Emission spectrum of Al plasmas, Ti plasma, and Au plasmas have been successfully recorded by using X-ray CCD camera. It is demonstrated experimentally that the measured wavelength is accorded with the theoretical value.

  18. Laser System for Photoelectron and X-Ray Production in the PLEIADES Compton Light Source

    CERN Document Server

    Gibson, David J; Betts, S; Crane, John; Jovanovic, Igor

    2005-01-01

    The PLEIADES (Picosecond Laser-Electron Interaction for the Dynamic Evaluation of Structures) facility provides tunable short x-ray pulses with energies of 30-140 keV and pulse durations of 0.3 - 5 ps by scattering an intense, ultrashort laser pulse off a 35-75 MeV electron beam. Synchronization of the laser and electron beam is obtained by using a photoinjector gun, and using the same laser system to generate the electrons and the scattering laser. The Ti:Sapphire, chirped pulse amplification based 500 mJ, 50 fs, 810 nm scattering laser and the similar 300 μJ, 5 ps, 266 nm photoinjector laser systems are detailed. Additionally, an optical parametric chirped pulse amplification (OPCPA) system is studied as a replacement for part of the scattering laser front end. Such a change would significantly simplify the set-up the laser system by removing the need for active switching optics, as well as increase the pre-pulse contrast ratio which will be important when part of the scattering laser is used as a...

  19. Dose properties of x-ray beams produced by laser-wakefield-accelerated electrons

    International Nuclear Information System (INIS)

    Kainz, K K; Hogstrom, K R; Antolak, J A; Almond, P R; Bloch, C D

    2005-01-01

    Given that laser wakefield acceleration (LWFA) has been demonstrated experimentally to accelerate electron beams to energies beyond 25 MeV, it is reasonable to assess the ability of existing LWFA technology to compete with conventional radiofrequency linear accelerators in producing electron and x-ray beams for external-beam radiotherapy. We present calculations of the dose distributions (off-axis dose profiles and central-axis depth dose) and dose rates of x-ray beams that can be produced from electron beams that are generated using state-of-the-art LWFA. Subsets of an LWFA electron energy distribution were propagated through the treatment head elements (presuming an existing design for an x-ray production target and flattening filter) implemented within the EGSnrc Monte Carlo code. Three x-ray energy configurations (6 MV, 10 MV and 18 MV) were studied, and the energy width ΔE of the electron-beam subsets varied from 0.5 MeV to 12.5 MeV. As ΔE increased from 0.5 MeV to 4.5 MeV, we found that the off-axis and central-axis dose profiles for x-rays were minimally affected (to within about 3%), a result slightly different from prior calculations of electron beams broadened by scattering foils. For ΔE of the order of 12 MeV, the effect on the off-axis profile was of the order of 10%, but the central-axis depth dose was affected by less than 2% for depths in excess of about 5 cm beyond d max . Although increasing ΔE beyond 6.5 MeV increased the dose rate at d max by more than 10 times, the absolute dose rates were about 3 orders of magnitude below those observed for LWFA-based electron beams at comparable energies. For a practical LWFA-based x-ray device, the beam current must be increased by about 4-5 orders of magnitude. (note)

  20. Spectroscopic analysis of sodium-bearing Z-pinch plasmas for their x-ray-laser pumping efficiency

    International Nuclear Information System (INIS)

    Apruzese, J.P.; Mehlman, G.; Davis, J.; Rogerson, J.E.; Scherrer, V.E.; Stephanakis, S.J.; Ottinger, P.F.; Young, F.C.

    1987-01-01

    Using axially resolved spectra, we have derived temperature and density profiles of sodium-bearing Z-pinch plasmas produced on the Naval Research Laboratory's Gamble-II generator. The variations in the output power of the Na X 1s 2 1 S 0 --1s2p 1 P 1 line which can be used to pump a Ne IX x-ray laser, are analyzed as functions of mass loading, temperature, and density. The fractional conversion of plasma energy to lasing lines is projected as 10/sup -3/ if an optimum neon lasant plasma can be prepared and pumped to saturation. This would require an increase in load current of less than or equal to 50% from the present 1.2 MA