Radioactivity Handbook

International Nuclear Information System (INIS)

Firestone, R.B.; Browne, E.

1985-01-01

The Radioactivity Handbook will be published in 1985. This handbook is intended primarily for applied users of nuclear data. It will contain recommended radiation data for all radioactive isotopes. Pages from the Radioactivity Handbook for A = 221 are shown as examples. These have been produced from the LBL Isotopes Project extended ENDSF data-base. The skeleton schemes have been manually updated from the Table of Isotopes and the tabular data are prepared using UNIX with a phototypesetter. Some of the features of the Radioactivity Handbook are discussed here

Problems in producing nuclear reactor for medical isotopes and the Global Crisis of molybdenum supply

International Nuclear Information System (INIS)

Zubiarrain, A.

2011-01-01

Nuclear medicine uses drugs that incorporate a radioactive isotope radiopharmaceuticals. Every year are performed, worldwide, 35 million nuclear medicine procedures, of which 80% are done with radiopharmaceuticals containing the isotope, molybdenum-99, produced in nuclear reactors. In recent years, there have been several supply crisis of molybdenum-99, which have hampered diagnostic procedure with technitium-99m. (Author)

Radioactivity monitoring of Irish dairy produce

International Nuclear Information System (INIS)

Kelleher, K.

2010-01-01

Full text: The RPII has been carrying out monitoring of milk and dairy produce since 1986. Milk samples are routinely analysed for radiocaesium and strontium-90 as part of the RPII's environmental monitoring programme to determine the doses received to the Irish population from milk consumption. The method the RPII utilises for determining the Sr-90 activity in milk is by measuring the Cerenkov radiation produced by its daughter 90 Y isolated from interfering nuclides such as uranium, thorium, radium and their decay products as well as isotopes of caesium, potassium and strontium by extraction with 10% di-(2-ethylhexyl)phosphate (HDEHP) in toluene. The chemical yield of 90 Y is determined by the acidmetric titration of yttrium nitrate carrier with titriplex III. The levels of Sr-90 and dose to the Irish population from milk consumption have been negligible when compared to other radioactive sources in the Irish environment. Other dairy products are analysed for radiocaesium on a routine basis for commercial customers to ensure the levels of radioactivity in the dairy products fall within EC regulations governing the export/import of dairy produce. The export of milk and milk produce from Ireland is a very important industry, 80% of dairy products produced in Ireland are exported and these exports are worth Euro 2.2 billion annually to the Irish economy. The dairy products are analysed by gamma spectroscopy and include full and skim milk powders, butter, casein, cheese, cream, whey and lactose. The levels of radiocaesium in these products are typically below 5 Bk/kg and fall well within the limit of 370 Bq/kg laid down by the European Community in Council Regulation 737/90. Although the levels of these radionuclides are relatively low the RPII recognises the importance of analysing these samples for radioactivity to inform the public, ensure consumer confidence and, more importantly, to maintain a level of expertise in the RPII in these analytical techniques so that

Radioactivity monitoring of Irish dairy produce

Energy Technology Data Exchange (ETDEWEB)

Kelleher, K. (Radiological Protection Institute of Ireland. Radiation Monitoring, Dublin (Ireland))

2010-03-15

Full text: The RPII has been carrying out monitoring of milk and dairy produce since 1986. Milk samples are routinely analysed for radiocaesium and strontium-90 as part of the RPII's environmental monitoring programme to determine the doses received to the Irish population from milk consumption. The method the RPII utilises for determining the Sr-90 activity in milk is by measuring the Cerenkov radiation produced by its daughter 90Y isolated from interfering nuclides such as uranium, thorium, radium and their decay products as well as isotopes of caesium, potassium and strontium by extraction with 10% di-(2-ethylhexyl)phosphate (HDEHP) in toluene. The chemical yield of 90Y is determined by the acidmetric titration of yttrium nitrate carrier with titriplex III. The levels of Sr-90 and dose to the Irish population from milk consumption have been negligible when compared to other radioactive sources in the Irish environment. Other dairy products are analysed for radiocaesium on a routine basis for commercial customers to ensure the levels of radioactivity in the dairy products fall within EC regulations governing the export/import of dairy produce. The export of milk and milk produce from Ireland is a very important industry, 80% of dairy products produced in Ireland are exported and these exports are worth Euro 2.2 billion annually to the Irish economy. The dairy products are analysed by gamma spectroscopy and include full and skim milk powders, butter, casein, cheese, cream, whey and lactose. The levels of radiocaesium in these products are typically below 5 Bk/kg and fall well within the limit of 370 Bq/kg laid down by the European Community in Council Regulation 737/90. Although the levels of these radionuclides are relatively low the RPII recognises the importance of analysing these samples for radioactivity to inform the public, ensure consumer confidence and, more importantly, to maintain a level of expertise in the RPII in these analytical techniques so

TRI mu P - a radioactive isotope trapping facility under construction at KVI

CERN Document Server

Berg, G P; Dermois, O; Harakeh, M N; Hoekstra, R; Jungmann, Klaus; Kopecky, S; Morgenstern, R; Rogachevskiy, A; Timmermans, R; Willmann, L; Wilschut, H W

2003-01-01

At the Kernfysisch Versneller Instituut a new facility (TRI mu P) is under development which aims to investigate fundamental interactions using radioactive ions. A spectrum of radioactive isotopes will be produced in inverse-kinematics and fragmentation reactions using heavy-ion beams from the superconducting cyclotron AGOR. The reaction products will be separated from the primary beam in a dual-mode recoil and fragment separator. The beam of isotopes of interest will be transformed into a low-energy, high-quality, bunched beam and, after neutralization, stored in an atom trap. The emphasis will be put on studying the origin of parity violation via beta-nu angular correlations and the search for permanent electric dipole moments of atoms and nuclei. The facility will be open to outside users; suggestions for collaborations to extend the scientific program are encouraged.

Proton Radioactivity Measurements at HRIBF: Ho, Lu, and Tm Isotopes

International Nuclear Information System (INIS)

Akovali, Y.; Batchelder, J.C.; Bingham, C.R.; Davinson, T.; Ginter, T.N.; Gross, C.J.; Grzywacz, R.; Hamilton, J.H.; Janas, Z.; Karny, M.; Kim, S.H.; MacDonald, B.D.; Mas, J.F.; McConnell, J.W.; Piechaczek, A.; Ressler, J.J.; Rykaczewski, K.; Slinger, R.C.; Szerypo, J.; Toth, K.S.; Weintraub, W.; Woods, P.J.; Yu, C.-H.; Zganjar, E.F.

1998-01-01

Two new isotopes, 145 Tm and 140 Ho and three isomers in previously known isotopes, 141m Ho, 150m Lu and 151m Lu have been discovered and studied via their decay by proton emission. These proton emitters were produced at the Holifield Radioactive Ion Beam Facility (HRIBF) by heavy-ion fusion-evaporation reactions, separated in A/Q with a recoil mass spectrometer (RMS), and detected in a double-sided silicon strip detector (DSSD). The decay energy and half-life was measured for each new emitter. An analysis in terms of a spherical shell model is applied to the Tm and Lu nuclei, but Ho is considerably deformed and requires a collective model interpretation

Rechargeable radioactive isotope generator

International Nuclear Information System (INIS)

Thornton, A.K.; Cerone, F.E.

1978-01-01

The description is given of a rechargeable radioactive isotope generator having the following features: a box containing a transport shield, a shielded generator including elements for the absorption and holding of the parent isotope, an eluant tank, a first pipe causing this tank to communicate with the transport shield, a second pipe causing this transport shield to communicate with the shielded generator and a third pipe placing the shielded generator in communication with the outside of the unit. It also includes a shelf across the external front part of the unit a part of which is shielded by external components, a shielded elution flask in which the eluate is poured and a filter set at a point between the flask and the third pipe [fr

Uses of Radioactive Isotopes in Industry

International Nuclear Information System (INIS)

Plata, A.; Val Cob, M. del; Gamboa, J. M.

1962-01-01

The present report contains a list of some of the most important problems in industry that have been approached so far by the use of radioactive isotopes. The list has been compiled trough the experience gained by the authors in revising for several years the most important scientific journal and other sources of information on this subject. The classification of industries has been done in an arbitrary way, choosing those isotope uses that have reached a higher degree of development. (Author)

CERN: Producing radioactive beams

International Nuclear Information System (INIS)

Anon.

1994-01-01

Accelerating radioactive beams has long been of interest at CERN's ISOLDE on-line isotope separator - the possibility was discussed at a CERN Workshop on intermediate energy physics as early as 1977. Meanwhile, as was highlighted in the 1991 report of the Nuclear Physics European Collaboration Committee, widespread scientific interest in these beams has developed and a range of projects are proposed, under construction or operational throughout the world

Natural radioactive isotopes in food of Polish population

International Nuclear Information System (INIS)

Pietrzak-Lis, Z.

1999-01-01

The natural radioactive isotopes contamination of basic food products and water in two regions of Poland (Central Poland and Silesia Region) have been measured. The following isotopes have been taken into account: U-234, U-238, Th-228, Th-230, Th-232, Ra-226, Ra-228, Pb-210; Po-210. The annually intake of mentioned isotopes by regional population and relative doses have been assessed for typical diet of adults in Poland

A densimeter with radioactive isotope of teaching

International Nuclear Information System (INIS)

Qu Guopu; Zhao Xiuliang; Cheng Pinjing

2002-01-01

A densimeter with radioactive isotope beseemed experiment teaching for speciality of nuclear engineering and nuclear technology in higher education is presented. Principle of work and composing of instrument system are introduced briefly

Radioactive isotope and isomer separation with using light induced drift effect

International Nuclear Information System (INIS)

Hradecny, C.; Slovak, J.; Tethal, T.; Ermolaev, I.M.; Shalagin, A.M.

1991-01-01

The isotope separation with using light induced drift (LID) is discussed. The basic theoretical characteristics of the method are deduced: separation simultaneously with an arbitrary high enrichment and without significant losses; separation productivity up to 100 μg/h. These characteristics are sufficient and very convenient for separation of expensive radioactive isotopes and isomers which are applied in medicine and science. The first experimental separation of the radioactive isotopes ( 22,24 Na) by using the LID effect is reported. 13 refs.; 5 figs

Dynamics of radioactive lead isotopes in the global environmental atmosphere

International Nuclear Information System (INIS)

Koike, Yuya; Kosako, Toshiso

2006-01-01

Fundamental information of radioactive lead isotopes, which used as the atmospheric tracer in the global environmental atmosphere, is reviewed. Emanation and exhalation of Rn and Tn, parent nuclide, is stated. Some reports on measurement and application of short-lived lead isotopes are reported. Transfer of radioactive lead isotopes in the atmosphere, vertical profiles of radon, thoron, and short-lived lead isotopes for different turbulent mixing conditions, deposition to aerosol, basic processes of Rn decay product behavior in air defining 'unattached' and 'aerosol-attached' activities, seasonal variation of atmospheric 210 Pb concentration at Beijing and Chengdu, seasonal variation of atmospheric 212 Pb concentration at several observation sites in Japan Islands, and variation in the atmospheric concentration of 212 Pb along with SO 2 are shown. (S.Y.)

Characterization of defects in semiconductors using radioactive isotopes

CERN Document Server

Deicher, Manfred

2007-01-01

Radioactive atoms have been used in solid-state physics and in material science for many decades. Besides their classical application as tracer for diffusion studies, nuclear techniques such as Mossbauer spectroscopy, perturbed angular correlation, and emission channeling have used nuclear properties to gain microscopical information on the structural and dynamical properties of solids. The availability of many different radioactive isotopes as a clean ion beam at facilities like ISOLDE/CERN has triggered a new era involving methods sensitive for the optical and electronic properties of solids, especially in the field of semiconductor physics. Spectroscopic techniques like photoluminescence (PL), deep-level transient spectroscopy (DLTS), and Hall effect gain a new quality by using radioactive isotopes. Due to their decay the chemical origin of an observed electronic and optical behavior of a specific defect or dopant can be unambiguously identified. This contribution will highlight a few examples to illustrat...

Dating of oilfield contamination by Natural Occurring Radioactive Materials (NORM) using isotopic ratios

International Nuclear Information System (INIS)

Al-Masri, M. S.; Othman, I.; Aba, A.

2008-05-01

In the present work, the possibility of using radium isotope ratios (226, 224, 228) for dating of NORM contaminated sites in the oilfields due to uncontrolled disposal of produced water into the environmental NORM contaminated soil sample were collected from different locations in Syrian Oilfields and radioactivity analysed. In addition, production water samples were collected and analysed to determine the isotopes ratios of the naturally occurring radioactive materials. The results have shown that the 228 Ra/ 226 Ra can be successfully used to date contaminated soil provided that this ratio is determined in production water. Moreover, the 210 Pb/ 226 Ra activity ratios was used for the first time for dating of contaminated soil where all factors affecting the method application have been evaluated. Furthermore, the obtained results for dating using the three methods were compared with the actual contamination dates provided by the oil companies. (Authors)

Wide-band digital equipment for study of neutron reactions producing short-living isotopes

International Nuclear Information System (INIS)

Bonyushkin, E.K.; Boyarintsev, V.A.; Goryushkin, S.I.; Drozdov, Yu.M.; Orlov, R.A.

1976-01-01

Digital equipment designed for recording automatically curves of decay for radioactive isotopes with a half-life period of about 10 Ms is described. Detection of a signal produced by isotope-isomer radioactive radiation is performed in the integral mode. A block-diagram of the measuring channel corresponding to the current mode of recording is presented. The accuracy characteristics of such a measuring channel are determined primarily by parameters of an analog-digital converter and they do not depend upon the length of the signal cable. Principles of operation for digital equipment are based on logarithmic conversion of the d.c. voltage into a number of pulses by the oscillating contour, i.e. a number of pulses in the envelope is proportional to the logarithm of the strobbed voltage. The amplitude range of recording is higher than 10 3 . Total instrumental errors of recording are about 5 per cent

Safe handling of radioactive isotopes. Handbook 42

Energy Technology Data Exchange (ETDEWEB)

NONE

1949-09-15

With the increasing use of radioactive isotopes by industry, the medical profession, and research laboratories, it is essential that certain minimal precautions be taken to protect the users and the public. The recommendations contained in this handbook represent what is believed to be the best available opinions on the subject as of this date. As our experience with radioisotopes broadens, we will undoubtedly be able to improve and strengthen the recommendations for their safe handling and utilization. Through the courtesy of the National Research Council about a year ago, several hundred draft copies of this report were circulated to all leading workers and authorities in the field for comment and criticism. The present handbook embodies all pertinent suggestions received from these people. Further comment will be welcomed by the committee. One of the greatest difficulties encountered in the preparation of this handbook lay in the uncertainty regarding permissible radiation exposure levels - particularly for ingested radioactive materials. The establishment of sound figures for such exposure still remains a problem of high priority for many conditions and radioactive substances. Such figures as are used in this report represent the best available information today. If, in the future, these can be improved upon, appropriate corrections will be issued. The subject will be under continuous study by the two subcommittees mentioned above. The present Handbook has been prepared by the Subcommittee on the Handling of Radioactive Isotopes and Fission Products.

Safe handling of radioactive isotopes. Handbook 42

International Nuclear Information System (INIS)

1949-09-01

With the increasing use of radioactive isotopes by industry, the medical profession, and research laboratories, it is essential that certain minimal precautions be taken to protect the users and the public. The recommendations contained in this handbook represent what is believed to be the best available opinions on the subject as of this date. As our experience with radioisotopes broadens, we will undoubtedly be able to improve and strengthen the recommendations for their safe handling and utilization. Through the courtesy of the National Research Council about a year ago, several hundred draft copies of this report were circulated to all leading workers and authorities in the field for comment and criticism. The present handbook embodies all pertinent suggestions received from these people. Further comment will be welcomed by the committee. One of the greatest difficulties encountered in the preparation of this handbook lay in the uncertainty regarding permissible radiation exposure levels - particularly for ingested radioactive materials. The establishment of sound figures for such exposure still remains a problem of high priority for many conditions and radioactive substances. Such figures as are used in this report represent the best available information today. If, in the future, these can be improved upon, appropriate corrections will be issued. The subject will be under continuous study by the two subcommittees mentioned above. The present Handbook has been prepared by the Subcommittee on the Handling of Radioactive Isotopes and Fission Products

Radiological impact assessment of the domestic on-road transportation of radioactive isotope wastes

Energy Technology Data Exchange (ETDEWEB)

Seo, Myung Hwan; Hong, Sung Wook; Park, Jin Beak [Korea Radioactive Waste Agency, Technology Institute, Daejeon (Korea, Republic of)

2016-09-15

Korea Radioactive Waste Agency (KORAD) began to operate the low and intermediate level radioactive waste disposal facility in Gyeongju and to transport the radioactive waste containing radioactive isotopes from Daejeon to the disposal facility for the first time at 2015. For this radioactive waste transportation, in this study, radiological impact assessment is carried out for workers and public. The dose rate to workers and public during the transportation is estimated with consideration of the transportation scenarios and is compared with the Korean regulatory limit. The sensitivity analysis is carried out by considering both the variation of release ratios of the radioactive isotopes from the waste and the variation of the distances between the radioactive waste drum and worker during loading and unloading of radioactive waste. As for all the transportation scenarios, radiological impacts for workers and public have met the regulatory limits.

The containment and an absorbent evaluation for a package for a liquid radioactive isotope

Energy Technology Data Exchange (ETDEWEB)

Bang, K. S.; Lee, J. C.; Kim, D. H.; Hwang, C. S.; Kim, H. J.; Seo, K. S

2005-03-01

Radioactive isotopes must be safely transported from the production centre to the point of use. The shipping package to safely transport radioactive isotopes should be able to withstand the conditions prescribed by law. A type a package, which is used to transport liquid radioactive materials, should have a containment system comprising a primary inner and a secondary outer containment or it should be provided with a sufficiently absorbent material to absorb twice the volume of the liquid contents. Accordingly, an absorbent material for use in a Type A package to transport a liquid radioactive isotope was estimated. To estimate the integrity of containment, the leakage tests for a containment system for a Type A package for domestic and abroad expert were conducted.

Novel methods for estimating 3D distributions of radioactive isotopes in materials

Energy Technology Data Exchange (ETDEWEB)

Iwamoto, Y., E-mail: y.iwamoto0805@ruri.waseda.jp [Research Institute for Science and Engineering, Waseda University, Shinjuku, Tokyo 169-8555 (Japan); Kataoka, J.; Kishimoto, A.; Nishiyama, T.; Taya, T.; Okochi, H.; Ogata, H. [Research Institute for Science and Engineering, Waseda University, Shinjuku, Tokyo 169-8555 (Japan); Yamamoto, S. [Nagoya University Graduate School of Medicine, 1-1-20, Daikominami, Higashi-ku, Nagoya-shi, Aichi 461-8673 (Japan)

2016-09-21

In recent years, various gamma-ray visualization techniques, or gamma cameras, have been proposed. These techniques are extremely effective for identifying “hot spots” or regions where radioactive isotopes are accumulated. Examples of such would be nuclear-disaster-affected areas such as Fukushima or the vicinity of nuclear reactors. However, the images acquired with a gamma camera do not include distance information between radioactive isotopes and the camera, and hence are “degenerated” in the direction of the isotopes. Moreover, depth information in the images is lost when the isotopes are embedded in materials, such as water, sand, and concrete. Here, we propose two methods of obtaining depth information of radioactive isotopes embedded in materials by comparing (1) their spectra and (2) images of incident gamma rays scattered by the materials and direct gamma rays. In the first method, the spectra of radioactive isotopes and the ratios of scattered to direct gamma rays are obtained. We verify experimentally that the ratio increases with increasing depth, as predicted by simulations. Although the method using energy spectra has been studied for a long time, an advantage of our method is the use of low-energy (50–150 keV) photons as scattered gamma rays. In the second method, the spatial extent of images obtained for direct and scattered gamma rays is compared. By performing detailed Monte Carlo simulations using Geant4, we verify that the spatial extent of the position where gamma rays are scattered increases with increasing depth. To demonstrate this, we are developing various gamma cameras to compare low-energy (scattered) gamma-ray images with fully photo-absorbed gamma-ray images. We also demonstrate that the 3D reconstruction of isotopes/hotspots is possible with our proposed methods. These methods have potential applications in the medical fields, and in severe environments such as the nuclear-disaster-affected areas in Fukushima.

Novel methods for estimating 3D distributions of radioactive isotopes in materials

Science.gov (United States)

Iwamoto, Y.; Kataoka, J.; Kishimoto, A.; Nishiyama, T.; Taya, T.; Okochi, H.; Ogata, H.; Yamamoto, S.

2016-09-01

In recent years, various gamma-ray visualization techniques, or gamma cameras, have been proposed. These techniques are extremely effective for identifying "hot spots" or regions where radioactive isotopes are accumulated. Examples of such would be nuclear-disaster-affected areas such as Fukushima or the vicinity of nuclear reactors. However, the images acquired with a gamma camera do not include distance information between radioactive isotopes and the camera, and hence are "degenerated" in the direction of the isotopes. Moreover, depth information in the images is lost when the isotopes are embedded in materials, such as water, sand, and concrete. Here, we propose two methods of obtaining depth information of radioactive isotopes embedded in materials by comparing (1) their spectra and (2) images of incident gamma rays scattered by the materials and direct gamma rays. In the first method, the spectra of radioactive isotopes and the ratios of scattered to direct gamma rays are obtained. We verify experimentally that the ratio increases with increasing depth, as predicted by simulations. Although the method using energy spectra has been studied for a long time, an advantage of our method is the use of low-energy (50-150 keV) photons as scattered gamma rays. In the second method, the spatial extent of images obtained for direct and scattered gamma rays is compared. By performing detailed Monte Carlo simulations using Geant4, we verify that the spatial extent of the position where gamma rays are scattered increases with increasing depth. To demonstrate this, we are developing various gamma cameras to compare low-energy (scattered) gamma-ray images with fully photo-absorbed gamma-ray images. We also demonstrate that the 3D reconstruction of isotopes/hotspots is possible with our proposed methods. These methods have potential applications in the medical fields, and in severe environments such as the nuclear-disaster-affected areas in Fukushima.

Review of Cyclotrons for the Production of Radioactive Isotopes for Medical and Industrial Applications

Science.gov (United States)

Schmor, Paul

2011-02-01

Radioactive isotopes are used in a wide range of medical, biological, environmental and industrial applications. Cyclotrons are the primary tool for producing the shorter-lived, proton-rich radioisotopes currently used in a variety of medical applications. Although the primary use of the cyclotron-produced short-lived radioisotopes is in PET/CT (positron emission tomography/computed tomography) and SPECT (single photon emission computed tomography) diagnostic medical procedures, cyclotrons are also producing longer-lived isotopes for therapeutic procedures as well as for other industrial and applied science applications. Commercial suppliers of cyclotrons are responding by providing a range of cyclotrons in the energy range of 3-70MeV for the differing needs of the various applications. These cyclotrons generally have multiple beams servicing multiple targets. This review article presents some of the applications of the radioisotopes and provides a comparison of some of the capabilities of the various current cyclotrons. The use of nuclear medicine and the number of cyclotrons supplying the needed isotopes are increasing. It is expected that there will soon be a new generation of small "tabletop" cyclotrons providing patient doses on demand.

Reduction of radioactivity produced by nuclear explosives

Energy Technology Data Exchange (ETDEWEB)

Lessler, Richard M [Lawrence Radiation Laboratory, University of California, Livermore, CA (United States)

1970-05-15

Four main sources contribute to the radioactivity produced by a nuclear explosive: 1. Fission products from the nuclear explosive, 2. Fusion products from the nuclear explosive, 3. Induced radioactivity in the nuclear explosive, 4. Induced radioactivity in the environment. This paper will summarize some of the work done at the Lawrence Radiation Laboratory at Livermore to reduce the radioactivity from these sources to levels acceptable for peaceful applications. Although it is theoretically possible to have no radioactivity produced by nuclear explosives, this goal has not been achieved.

Decoding Environmental Processes Using Radioactive Isotopes for the Post-Radioactive Contamination Recovery Assessment

Science.gov (United States)

Yasumiishi, Misa; Nishimura, Taku; Osawa, Kazutoshi; Renschler, Chris

2017-04-01

The continual monitoring of environmental radioactive levels in Fukushima, Japan following the nuclear plant accident in March 2011 provides our society with valuable information in two ways. First, the collected data can be used as an indicator to assess the progress of decontamination efforts. Secondly, the collected data also can be used to understand the behavior of radioactive isotopes in the environment which leads to further understanding of the landform processes. These two aspects are inseparable for us to understand the effects of radioactive contamination in a dynamic environmental system. During the summer of 2016, 27 soil core samples were collected on a farmer's land (rice paddies and forest) in Fukushima, about 20 km northwest of the nuclear plant. Each core was divided into 2.0 - 3.0 cm slices for the Cs-134, Cs-137, and I-131 level measurement. The collected data is being analyzed from multiple perspectives: temporal, spatial, and geophysical. In the forest area, even on the same hillslope, multiple soil types and horizon depths were observed which indicates the challenges in assessing the subsurface radioactive isotope movements. It appears that although highly humic soils show higher or about the same level of radioactivity in the surface layers, as the depth increased, the radioactivity decreased more in those samples compared with more sandy soils. With regard to the direction a slope faces and the sampling altitudes, the correlation between those attributes and radioactivity levels is inconclusive at this moment. The altitude might have affected the fallout level on a single hillslope-basis. However, to determine the correlation, further sampling and the detailed analysis of vegetation and topography might be necessary. Where the surface soil was scraped and new soil was brought in, former rice paddy surface layers did show three-magnitude levels lower of radioactivity in the top layer when compared with forest soils. At the foot of forest

Method of producing radioactive carbon powder

International Nuclear Information System (INIS)

Imamura, Y.

1980-01-01

Carbon powder, placed in a hermetically closed apparatus under vacuum together with radium ore, adsorbs radon gas emanating from the radium ore thus producing a radioactive carbonaceous material, the radioactivity of which is due to the presence of adsorbed radon. The radioactive carbon powder thus obtained has excellent therapeutical efficacy and is suitable for a variety of applications because of the mild radioactivity of radon. Radium ore permits substantially limitlessly repeated production of the radioactive carbon powder

Therapeutic use of radioactive isotopes

CERN Document Server

Caroline Duc

2013-01-01

In December, researchers from ISOLDE-CERN, the Paul Scherrer Institute (PSI) and the Institut Laue-Langevin (ILL) published the results of an in vivo study which successfully proved the effectiveness of four terbium isotopes for diagnosing and treating cancerous tumours.   Four terbium isotopes suitable for clinical purposes. “ISOLDE is the only installation capable of supplying terbium isotopes of such purity and intensity in the case of three out of the four types used in this study,” explains Karl Johnson, a physicist at ISOLDE.  “Producing over a thousand different isotopes, our equipment offers the widest choice of isotopes in the world!” Initially intended for fundamental physics research, ISOLDE has diversified its activities over time to invest in various projects in the materials science, biochemistry and nuclear medicine fields. The proof-of-concept study has confirmed that the four terbium isotopes 149Tb, 152Tb, 155Tb produ...

Process for improving the separation efficiency in the isolation of radioactive isotopes in elementary or chemically bonded form from liquids and gases

International Nuclear Information System (INIS)

Schmidberger, R.; Kirch, R.; Kock, W.

1986-01-01

In the process for the improvement of the separation efficiency in the isolation of radioactive isotopes in elementary or chemically bonded form from liquids or gases by ion exchange and adsorption, non-radioactive isotopes of the element to be isolated are added to the fluid before the isolation, whereas at the same time a large surplus of the non-radioactive isotopes to the radioactive isotopes is achieved by addition of only small quantities of compounds of the non-radioactive isotopes. (orig./RB) [de

Radioactive isotopes in clinical medicine and research. Abstracts

International Nuclear Information System (INIS)

2007-01-01

The review on the International Symposium on radioactive isotopes in clinical medicine and research in Bad Hofgastein, Austria, 9-12 January 2008, contains 42 papers and 29 poster contributions on the following topics: radiopharmaceutical sciences; radiopharmaceutical sciences in oncology and cardiology; therapy; endocrinology; molecular imaging; clinical PET; physics: image processing; instrumentation, neurology, psychiatry

Radioactive isotopes in clinical medicine and research. Abstracts

Energy Technology Data Exchange (ETDEWEB)

NONE

2007-07-01

The review on the International Symposium on radioactive isotopes in clinical medicine and research in Bad Hofgastein, Austria, 9-12 January 2008, contains 42 papers and 29 poster contributions on the following topics: radiopharmaceutical sciences; radiopharmaceutical sciences in oncology and cardiology; therapy; endocrinology; molecular imaging; clinical PET; physics: image processing; instrumentation, neurology, psychiatry.

Artificial neural network application in isotopic characterization of radioactive waste drums

International Nuclear Information System (INIS)

Potiens Junior, Ademar Jose

2005-01-01

One of the most important aspects to the development of the nuclear technology is the safe management of the radioactive waste arising from several stages of the nuclear fuel cycles, as well as from production and use of radioisotope in the medicine, industry and research centers. The accurate characterization of this waste is not a simple task, given to its diversity in isotopic composition and non homogeneity in the space distribution and mass density. In this work it was developed a methodology for quantification and localization of radionuclides not non homogeneously distributed in a 200 liters drum based in the Monte Carlo Method and Artificial Neural Network (RNA), for application in the isotopic characterization of the stored radioactive waste at IPEN. Theoretical arrangements had been constructed involving the division of the radioactive waste drum in some units or cells and some possible configurations of source intensities. Beyond the determination of the detection positions, the respective detection efficiencies for each position in function of each cell of the drum had been obtained. After the construction and the training of the RNA's for each developed theoretical arrangement, the validation of the method were carried out for the two arrangements that had presented the best performance. The results obtained show that the methodology developed in this study could be an effective tool for isotopic characterization of radioactive wastes contained in many kind of packages. (author)

A new class of medicament: radioactivity isotopes (1962)

International Nuclear Information System (INIS)

Cohen, Y.

1962-01-01

Very many radioelement are used in medicine, either for diagnosis or as therapeutics. The development of medicine has entailed an increase in the number of application of radioactive isotopes. Firstly used in the form of simple inorganic molecules for diagnosis or as anticancer therapeutics, radioelements are now used for labelling organic molecules, allowing functional specific studies of any kind of nature. Their production is made difficult by their radio-active properties. Their pharmaceutical properties, determined by tests and controls, depend either from radiochemistry and from medicine. The author reminds, in this report, the methods for the preparation and analysis, and set out the medical application. (author) [fr

Techniques to produce and accelerate radioactive ion beams

CERN Document Server

Penescu, Liviu Constantin; Lettry, Jacques; Cata-Danil, Gheorghe

The production and acceleration of the Radioactive Ion Beams (RIB) continues the long line of nuclear investigations started in the XIXth century by Pierre and Marie Curie, Henri Becquerel and Ernest Rutherford. The contemporary applications of the RIBs span a wide range of physics fields: nuclear and atomic physics, solid-state physics, life sciences and material science. ISOLDE is a world-leading Isotope mass-Separation On-Line (ISOL) facility hosted at CERN in Geneva for more than 40 years, offering the largest variety of radioactive ion beams with, until now, more than 1000 isotopes of more than 72 elements (with Z ranging from 2 to 88), with half-lives down to milliseconds and intensities up to 1011 ions/s. The post acceleration of the full variety of beams allows reaching final energies between 0.8 and 3.0 MeV/u. This thesis describes the development of a new series of FEBIAD (“Forced Electron Beam Induced Arc Discharge”) ion sources at CERN-ISOLDE. The VADIS (“Versatile Arc Discharge Ion Source�...

Radioactive isotopes are use wide in medicine

International Nuclear Information System (INIS)

Vargas, Celso

2011-01-01

The radioactive isotopes are used in medicine to view the status of an organ under different conditions; especially in the evolution of an organism after treatment of a cancer. In this process, three key areas have combined; first, the production of isotopes by developing of accelerators or reactors both linear accelerator and cyclotrons. Second, the use of suitable equipment such as PET (Positron emission tomography) for accurate scan of internal organs at physiological and biochemical level or molecular for diagnosis and effective treatment of diseases such as cancer. Currently, the trend has been to combine PET with other technologies such as CAT (computed axial tomographic) or SPECT (Single photon emission computer tomography). Third and finally, the development of molecules increasingly specific that have allowed to obtain several chemical compounds for different uses [es

ISOL science at the Holifield Radioactive Ion Beam Facility

Energy Technology Data Exchange (ETDEWEB)

Beene, James R [ORNL; Bardayan, Daniel W [ORNL; Galindo-Uribarri, Alfredo {nmn} [ORNL; Gross, Carl J [ORNL; Jones, K. L. [University of Tennessee, Knoxville (UTK); Liang, J Felix [ORNL; Nazarewicz, Witold [ORNL; Stracener, Daniel W [ORNL; Tatum, B Alan [ORNL; Varner Jr, Robert L [ORNL

2011-01-01

The Holi eld Radioactive Ion Beam Facility, located in Oak Ridge, Tennessee, is operated as a National User Facility for the U.S. Department of Energy, producing high quality ISOL beams of short-lived, radioactive nuclei for studies of exotic nuclei, astrophysics research, and various societal applications. The primary driver, the Oak Ridge Isochronous Cyclotron, produces rare isotopes by bombarding highly refractory targets with light ions. The radioactive isotopes are ionized, formed into a beam, mass selected, injected into the 25-MV Tandem, accelerated, and used in experiments. This article reviews HRIBF and its science.

Kinetics of isotopic exchanges by using radioactive indicators

International Nuclear Information System (INIS)

May, S.

1958-12-01

After having noticed that iodine 131 under the form of sodium iodide has always been used as radioactive indicator in the CEA atomic pile located in Chatillon, this research report recalls the counting technique and some historical aspects of the notion of isotopic exchange and qualitative works, and presents some generalities on isotopic exchanges (reactions and calculation of rate constants of order 1 and 2, calculation of activation energy, spectro-photometric studies, Walden inversion, alkaline hydrolysis, influence of solvent on exchange kinetics, influence of the nature of the mineral halide). The author then addresses exchanges in aliphatic series (exchange with sodium iodide and with molecular iodine), exchanges in olefin series, exchanges in alicyclic series, and exchanges in aromatic series

A theoretical study of cluster radioactivity in platinum isotopes

Energy Technology Data Exchange (ETDEWEB)

Joseph, Deepthy Maria; Ashok, Nithu; Joseph, Antony [University of Calicut, Department of Physics, Malappuram, Kerala (India)

2018-01-15

The probable cluster decay modes in platinum isotopes are predicted with the help of effective liquid drop model. The calculated half-lives are compared with those of universal decay law model and with the experimental data. The investigation affirms the decisive role of neutron magicity in the phenomenon of cluster radioactivity. It is found that the probability of cluster emission decreases with the increase in the neutron number of parent nucleus. Geiger-Nuttall plots of the probable decay modes show linear behaviour, which in turn leads to the equation for logarithmic half-life for the clusters emitted from Pt isotopes. (orig.)

Isotope products manufacture in Russia and its prospects

International Nuclear Information System (INIS)

Malyshev, S.V.; Okhotina, I.A.; Kalelin, E.A.; Krasnov, N.N.; Kuzin, V.V.; Malykh, J.A.; Makarovsky, S.B.

1997-01-01

At the present stage of the world economy development, stable and radioactive isotopes,preparations and products on their base are widely used in many fields of the national economy, medicine and scientific researches. The Russian Federation is one of the largest worldwide producers of a variety of nuclide products on the base of more than 350 isotopes, as follows: stable isotopes reactor, cyclotron, fission product radioactive isotopes, ion-radiation sources compounds, labelled with stable and radioactive isotopes, radionuclide short-lived isotope generators, radiopharmaceuticals, radionuclide light and heat sources; luminous paints on base of isotopes. The Russian Ministry for Atomic Energy coordinates activity for development and organization of manufacture and isotope products supply in Russia as well as for export. Within many years of isotope industry development, there have appeared some manufacturing centres in Russia, dealing with a variety of isotope products. The report presents the production potentialities of these centres and also an outlook on isotope production development in Russia in the next years

Estimate of the intensities of the radioactive nuclides produced at the super-FRS at the future GSI facility

International Nuclear Information System (INIS)

Ricciardi, M.V.

2004-11-01

The principal goal of the new facility is the construction of a worldwide unique and technically innovative accelerator system that will provide an extensive range of particle beams. Proton and antiproton beams will be available and ion beams of all chemical elements up to uranium will be produced with world-record intensities. The main employ of the high-intensity ion beams is the production of energetic beams of short-lived (radioactive) nuclei, in the following referred to as exotic or Rare Isotope Beams (RIBs). RIBs are produced in nuclear reactions experienced by the primary beams of stable particles. We report on the study of the production of radioactive nuclides and of their propagation through the Super-FRS. The study was performed by means of a nuclear-reaction Monte-Carlo code, ABRABLA, opportunely implemented for the above-described purpose. This work offers an overview of the radioactivity production in the Super-FRS area; the latter is the required starting knowledge for the design of the shielding structure. (orig.)

RIKEN radioactive isotope beam factory project – Present status and ...

Indian Academy of Sciences (India)

Programs for studying nuclear reactions and structure of exotic nuclei available at the RIKEN radioactive isotope beam factory project are introduced and discussed by demonstrating recent highlights. Special emphasis ... RIKEN Nishina Center for Accelerator-Based Science, 2-1 Hirosawa, Wako, Saitama 351-0198, Japan ...

Study of the Production of Radioactive Isotopes through Cosmic Muon Spallation in KamLAND

Energy Technology Data Exchange (ETDEWEB)

KamLAND Collaboration; Abe, S.; Enomoto, S.; Furuno, K.; Gando, Y.; Ikeda, H.; Inoue, K.; Kibe, Y.; Kishimoto, Y.; Koga, M.; Minekawa, Y.; Mitsui, T.; Nakajima, K.; Nakajima, K.; Nakamura, K.; Nakamura, M.; Shimizu, I.; Shimizu, Y.; Shirai, J.; Suekane, F.; Suzuki, A.; Takemoto, Y.; Tamae, K.; Terashima, A.; Watanabe, H.; Yonezawa, E.; Yoshida, S.; Kozlov, A.; Murayama, H.; Busenitz, J.; Classen, T.; Grant, C.; Keefer, G.; Leonard, D. S.; McKee, D.; Piepke, A.; Banks, T. I.; Bloxham, T.; Detwiler, J. A.; Freedman, S. J.; Fujikawa, B. K.; Gray, F.; Guardincerri, E.; Hsu, L.; Ichimura, K.; Kadel, R.; Lendvai, C.; Luk, K.-B.; O' Donnell, T.; Steiner, H. M.; Winslow, L. A.; Dwyer, D. A.; Jillings, C.; Mauger, C.; McKeown, R. D.; Vogel, P.; Zhang, C.; Berger, B. E.; Lane, C. E.; Maricic, J.; Miletic, T.; Batygov, M.; Learned, J. G.; Matsuno, S.; Pakvasa, S.; Foster, J.; Horton-Smith, G. A.; Tang, A.; Dazeley, S.; Downum, K. E.; Gratta, G.; Tolich, K.; Bugg, W.; Efremenko, Y.; Kamyshkov, Y.; Perevozchikov, O.; Karwowski, H. J.; Markoff, D. M.; Tornow, W.; Heeger, K. M.; Piquemal, F.; Ricol, J.-S.; Decowski, M. P.

2009-06-30

Radioactive isotopes produced through cosmic muon spallation are a background for rare event detection in {nu} detectors, double-beta-decay experiments, and dark-matter searches. Understanding the nature of cosmogenic backgrounds is particularly important for future experiments aiming to determine the pep and CNO solar neutrino fluxes, for which the background is dominated by the spallation production of {sup 11}C. Data from the Kamioka Liquid scintillator Anti-Neutrino Detector (KamLAND) provides valuable information for better understanding these backgrounds, especially in liquid scintillator, and for checking estimates from current simulations based upon MUSIC, FLUKA, and Geant4. Using the time correlation between detected muons and neutron captures, the neutron production yield in the KamLAND liquid scintillator is measured to be (2.8 {+-} 0.3) x 10{sup -4} n/({mu} {center_dot} (g/cm{sup 2})). For other isotopes, the production yield is determined from the observed time correlation related to known isotope lifetimes. We find some yields are inconsistent with extrapolations based on an accelerator muon beam experiment.

International Isotopes Markets

Directory of Open Access Journals (Sweden)

Stanislaw Z. Zhiznin

2016-01-01

Full Text Available The paper studies world markets of stable and radioactive isotopes. Isotopes have found various applications in science, industry, agriculture and other sectors of the economy, but especially - in medicine. Nuclear medicine is developing intensively all over the world thanks to the success in the treatment of various diseases with the help of radioactive pharmaceuticals (radiopharmaceuticals. The article uses empirical data from a forecast study of the global radiopharmaceuticals market made in 2015 by a research company «Markets and Markets» for the European, North American and global markets. The paper also analyzes the statistical data on the global export and import of natural uranium, enriched and depleted uranium, plutonium, thorium and some stable isotopes of non-medical purposes, presented by a company «Trend economy» in 2014. Despite a unique industrial base for the production of isotopes created in the Soviet Union Russia occupies a modest position on the world market of nuclear medicine except for certain areas. More than 80% of isotopes, produced in USSR were consumed domestically, the export of the stable and radioactive isotopes was in equal proportions. Now the country's domestic radiopharmaceuticals market is poorly developed. To radically change the situation, it is necessary to carry out reforms that stimulate the development of nuclear medicine.

Treatment of radioactive effluents at the Boris Kidric Institute

International Nuclear Information System (INIS)

Bojovic, P.; Drobnik, S.; Popara, D.

1964-10-01

The paper describes the origin, composition and activity of radioactive effluents at the Boris Kidric Institute, their collection at the places or origin, transport to the place of disposal and treatment of some smaller quantities. Special attention has been paid to effluents with short-lived isotopes produced in the Laboratory for radioactive isotope production (author)

Preliminary economic feasibility study of MIP (Medical Isotopes Producer)

International Nuclear Information System (INIS)

Mon, G. H.; O, S. Y.

2004-01-01

Preliminary economic feasibility study of MIP (Medical Isotopes Producer), which is used liquid nuclear fuel to produce medical isotopes of Mo-99 and Sr-89, was performed. To do this, this study was estimated the IRR(Internal Rate of Return) and PBP(Pay-back Period) about optimistic and pessimistic cases for market penetration of Asia and U.S.A. isotope markets. And sensitivity analysis is also performed about capital cost and price of Mo-99 and Sr-89. According to the results, IRR was between 14.9% and 24.3%, and PBP was between 4.8 years and 7.8 years. These suggest that MIP has economic merits. MIP can produce other medical isotopes such as Sr-90, I-131, Xe-133, Cs-137. So, it is necessary to do cost-benefit analysis considering production of these other isotopes

Production of radioactive ion beams and resonance ionization spectroscopy with the laser ion source at on-line isotope separator ISOLDE

International Nuclear Information System (INIS)

Fedosseev, V.N.; )

2005-01-01

Full text: The resonance ionisation laser ion source (RILIS) of the ISOLDE on-line isotope separation facility at CERN is based on the method of laser step-wise resonance ionisation of atoms in a hot metal cavity. Using the system of dye lasers pumped by copper vapour lasers the ion beams of many different metallic elements have been produced at ISOLDE with an ionization efficiency of up to 27%. The high selectivity of the resonance ionization is an important asset for the study of short-lived nuclides produced in targets bombarded by the proton beam of the CERN Booster accelerator. Radioactive ion beams of Be, Mg, Al, Mn, Ni, Cu, Zn, Ga, Ag, Cd, In, Sn, Sb, Tb, Yb, Tl, Pb and Bi have been generated with the RILIS. Setting the RILIS laser in the narrow line-width mode provides conditions for a high-resolution study of hyperfine structure and isotopic shifts of atomic lines for short-lived isotopes. The isomer selective ionization of Cu, Ag and Pb isotopes has been achieved by appropriate tuning of laser wavelengths

Radioactive isotopes and radiation in South Africa: a bibliographic review

International Nuclear Information System (INIS)

Basson, J.K.

1985-12-01

The development of isotope applications has been a main theme of the erstwhile Atomic Energy Board which organized a national conference in Pretoria in 1963 'to take stock of the work done in the country so far'. Radioactive isotopes and radiation have achieved widespread use in all fields of medicine, agriculture, science and technology. It was recommended that the AEC publish a review of relevant South African work. This publication therefore consists of listings of available publications by South African-based scientists since the 1963 Conference and is divided into the four categories: radiotherapy, clinical and laboratory medicine, agriculture, and industry, preceded by overviews. The terms of reference were construed not to include stable isotopes and it was accordingly decided to concentrate only on radioisotope applications

Radioactive isotopes in clinical medicine and research. Abstracts

International Nuclear Information System (INIS)

2005-01-01

The contribution displays 44 abstracts and 35 posters from the 27th International Symposium on ''radioactive isotopes in clinical medicine and research'', organized by the Austrian society of nuclear medicine and the department of nuclear medicine and the center for biomedical engineering and physics of the Vienna medical university. The abstracts are sorted according to lecture headers: radiopharmaceutical sciences, endocrinology, clinical PET, neurology, oncology, physics and instrumentation, cardiology, inflammation, therapy and varia. (uke)

Public service of radioactive waste management for small producers

International Nuclear Information System (INIS)

Zeleznik, N.; Mele, I.

2001-01-01

By Governmental decree of May 1999, the Agency for radwaste management (ARAO) was authorized as a state public service for managing radioactive waste from small producers. By this decree the ARAO also became the operator of the Central Interim Storage intended for radioactive waste from industry, medicine and research, located in Brinje near Ljubljana. In this paper the current situation will be presented, together with plans for improving public service and the necessary refurbishment and modernization of the storage facility. Execution of the proposed measures, modifications and a modernization will ensure proper and safe storing of all radioactive waste from small producers produced in Slovenia, thus fulfilling the requirements for full operation of the public service of radioactive waste management.(author)

Tomogram forming process and apparatus using radioactive isotopes

International Nuclear Information System (INIS)

Stoddart, H.F.

1980-01-01

This invention relates to nuclear medicine and particularly to a tomogram forming apparatus which permits, with great efficiency, the very sensitive quantitative determination and the accurate spatial localization of the radioactivity of a body section of a patient to whom a substance labelled with radioactive isotopes has been administered. This scanner is characterized in that it includes several highly focused collimators placed one after the other, according to an arrangement which surrounds a scanning field. Each collimator is mobile with respect to the adjacent one and a system enables the arrangement to be rotated about the scanning field from one scanning position to another. Another device enables the collimators to be moved so that, for each scanning position, the focus of each collimator uniformly samples at least half the scanning field [fr

Resonant ionization by laser beams: application to ions sources and to study the nuclear structure of radioactive tellurium isotopes

International Nuclear Information System (INIS)

Sifi, R.

2007-07-01

The radioactive ion beams that are produced through current isotope separators are well separated according to the A mass but not according to the Z parameter. The resonant ionization through laser beams applied to ion sources allows the production of radioactive ion beam in a very selective and efficient way by eliminating the isobaric contamination. The first chapter is dedicated to the resonant ionization by laser beams, we describe the principle, the experimental setting, the lasers used, the ionization schemes and the domain of application. The second chapter deals with the application of resonant ionization to laser ion sources for the production of radioactive ion beams. We present experimental tests performed for getting copper ion beams. Resonant ionization through laser is also used in the spectroscopy experiments performed at the Isolde (isotope separation on-line device) installation in CERN where more than 20 elements are ionized very efficiently. The technique is based on a frequency scanning around the excitation transition of the atoms in order to probe the hyperfine structure. Laser spectroscopy allows the determination of the hyperfine structure as well as the isotopic shift of atoms. In the third chapter the method is applied to the spectroscopy of tellurium atoms. First, we define the 2 parameters on which the extraction is based: charge radius and nuclear moments, then we present several theoretical models that we have used to assess our experimental results. (A.C.)

Isotope Production Facility (IPF)

Data.gov (United States)

Federal Laboratory Consortium — The Los Alamos National Laboratory has produced radioactive isotopes for medicine and research since the mid 1970s, when targets were first irradiated using the 800...

Management of radioactive wastes produced by users of radioactive materials

International Nuclear Information System (INIS)

1985-01-01

This report is intended as a document to provide guidance for regulatory, administrative and technical authorities who are responsible for, or are involved in, planning, approving, executing and reviewing national waste management programmes related to the safe use of radioactive materials in hospitals, research laboratories, industrial and agricultural premises and the subsequent disposal of the radioactive wastes produced. It provides information and guidance for waste management including treatment techniques that may be available to establishments and individual users

A kinematic-based methodology for radiological protection: Runoff analysis to calculate the effective dose for internal exposure caused by ingestion of radioactive isotopes

Science.gov (United States)

Sasaki, Syota; Yamada, Tadashi; Yamada, Tomohito J.

2014-05-01

We aim to propose a kinematic-based methodology similar with runoff analysis for readily understandable radiological protection. A merit of this methodology is to produce sufficiently accurate effective doses by basic analysis. The great earthquake attacked the north-east area in Japan on March 11, 2011. The system of electrical facilities to control Fukushima Daiichi nuclear power plant was completely destroyed by the following tsunamis. From the damaged reactor containment vessels, an amount of radioactive isotopes had leaked and been diffused in the vicinity of the plant. Radiological internal exposure caused by ingestion of food containing radioactive isotopes has become an issue of great interest to the public, and has caused excessive anxiety because of a deficiency of fundamental knowledge concerning radioactivity. Concentrations of radioactivity in the human body and internal exposure have been studied extensively. Previous radiologic studies, for example, studies by International Commission on Radiological Protection(ICRP), employ a large-scale computational simulation including actual mechanism of metabolism in the human body. While computational simulation is a standard method for calculating exposure doses among radiology specialists, these methods, although exact, are too difficult for non-specialists to grasp the whole image owing to the sophistication. In this study, the human body is treated as a vessel. The number of radioactive atoms in the human body can be described by an equation of continuity, which is the only governing equation. Half-life, the period of time required for the amount of a substance decreases by half, is only parameter to calculate the number of radioactive isotopes in the human body. Half-life depends only on the kinds of nuclides, there are no arbitrary parameters. It is known that the number of radioactive isotopes decrease exponentially by radioactive decay (physical outflow). It is also known that radioactive isotopes

Decay studies of neutron-deficient lawrencium isotopes

International Nuclear Information System (INIS)

Antalic, S.; Saro, S.; Streicher, B.; Venhart, M.; Hessberger, F.P.; Ackermann, D.; Heinz, S.; Kindler, B.; Kojouharov, I.; Lommel, B.; Mann, R.; Hofmann, S.; Kuusiniemi, P.; Leino, M.; Nishio, K.; Sulignano, B.

2008-01-01

The radioactive decay of the isotopes 254-256 Lr and their daughter products was investigated by means of α, prompt α-γ and delayed conversion electron-γ coincidence spectroscopy. The isotopes were produced using the reaction 48 Ca+ 209 Bi. (orig.)

Transmutation of stable isotopes and deactivation of radioactive waste in growing biological systems

International Nuclear Information System (INIS)

Vysotskii, Vladimir I.; Kornilova, Alla A.

2013-01-01

Highlights: ► The phenomena of isotope transmutation in growing microbiological cultures were investigated. ► Transmutation in microbiological associations is 20 times more effective than in pure cultures. ► Transmutation of radioactive nuclei to stable isotopes in such associations was investigated. ► The most accelerated rate of Cs 137 to stable Ba 138 isotope transmutation was 310 days. ► “Microbiological deactivation” may be used for deactivation of Chernobyl and Fukushima areas. - Abstract: The report presents the results of qualifying examinations of stable and radioactive isotopes transmutation processes in growing microbiological cultures. It is shown that transmutation of stable isotopes during the process of growth of microbiological cultures, at optimal conditions in microbiological associations, is 20 times more effective than the same transmutation process in the form of “one-line” (pure) microbiological cultures. In the work, the process of direct, controlled decontamination of highly active intermediate lifetime and long-lived reactor isotopes (reactor waste) through the process of growing microbiological associations has been studied. In the control experiment (flask with active water but without microbiological associations), the “usual” law of nuclear decay applies, and the life-time of Cs 137 isotope was about 30 years. The most rapidly increasing decay rate, which occurred with a lifetime τ * ≈ 310 days (involving an increase in rate, and decrease in lifetime by a factor of 35 times) was observed in the presence of Ca salt in closed flask with active water contained Cs 137 solution and optimal microbiological association

Application of radioactive isotopes in the field of investigations of the means of transportation wear

International Nuclear Information System (INIS)

Gromann, Kh-D.

1979-01-01

The Station for governing of isotope technique ensures application of radioactive isotopes in the transport of the GDR. The main directions of the isotope application are investigations of wear and leaks. It is reported about the wear investigations performed on models and real structural elements at laboratory testing stands as well as on the real structural elements in the exploitation conditions. Special attention should be paid to the numerous measurements of wear of engines, rails and so on. Data and valuable results have been obtained about the problem of the short-term wear measurement. Measurements of leaks by means of radioactive isotopes application is used for investigations of the hermeticy of the refrigerator tronsport means, heating systems and clymatizing installations of the carriges as well as stationary installations. Then, measurements have been done of leaks in pipelines as well as determinations of their lacalization and intensity. General and specific advantages of separate methods are discussed [ru

Regolith history from cosmic-ray-produced isotopes

International Nuclear Information System (INIS)

Fireman, E.L.

1974-04-01

A statistical model is given for soil development relating meteoroid impacts on the moon to cosmic-ray-produced isotopes in the soil. By means of this model, the average lunar mass loss rate during the past 14 aeons is determined to be 170 g/sq cm aeon and the soil mixing rate to be approximately 200 cm/aeon from the gadolinium isotope data for the Apollo 15 and 16 drill stems. The isotope data also restrict the time variation of the meteoroid flux during the past 14 aeons. (U.S.)

Classification of radioactive wastes produced by the nuclear industry

International Nuclear Information System (INIS)

2013-01-01

This document first indicates the origins of radioactive wastes (mainly electronuclear industry), and the composition of spent fuel, and that only fission products and minor actinides are considered as radioactive wastes whereas uranium and plutonium can be used as new fuel after recycling. The classification of radioactive wastes is indicated in terms of radioactivity level and radionuclide half-life: high level (0.2 per cent of the total waste volume but 96 per cent of total waste radioactivity), medium level long life (3 per cent of volume, 4 per cent of radioactivity), low level long life (7 per cent of volume, 0.1 per cent of radioactivity), low and medium level and short life (63 per cent of volume and 0.02 per cent of radioactivity), very low level (27 per cent of volume and less than 0.01 per cent of radioactivity). An overview of radioactive waste processing and storage in France is presented for each category. Current and predicted volumes are indicated for each category. The main challenges are briefly addressed: spent fuel recycling, waste valorisation by fourth-generation reactors. Processing locations in France and in the World are indicated. Some key figures are provided: 2 kg of radioactive waste are produced per inhabitant and per year, and waste management costs represent 5 per cent of the total cost of produced electricity

Yields and spectroscopy of radioactive isotopes at LOHENGRIN and ISOLDE

CERN Document Server

Köster, U

1999-01-01

Yields of radioactive nuclei were measured at two facilities: the recoil separator LOHENGRIN at the Institut Laue Langevin in Grenoble and the on-line isotope separator ISOLDE at CERN in Geneva. At LOHENGRIN the yields of light charged particles were measured from thermal neutron induced ternary fission of several actinide targets: 233U, 235U, 239Pu, 241Pu and 245Cm. Thin targets are brought into a high neutron flux. The produced nuclei leave these with the recoil obtained in the fission reaction. They are measured at different energies and ionic charge states. After corrections for the experimental acceptance, the time behaviour of the fission rate and the ionic charge fraction, the yields are integrated over the kinetic energy distribution. Comparing these yields with the predictions of various ternary fission models shows that the most abundant nuclides are well reproduced. On the other hand the models overestimate significantly the production of more "exotic" nuclides with an extreme N/Z ratio. Therefore ...

Radioactive waste management

International Nuclear Information System (INIS)

Blomek, D.

1980-01-01

The prospects of nuclear power development in the USA up to 2000 and the problems of the fuel cycle high-level radioactive waste processing and storage are considered. The problems of liquid and solidified radioactive waste transportation and their disposal in salt deposits and other geologic formations are discussed. It is pointed out that the main part of the high-level radioactive wastes are produced at spent fuel reprocessing plants in the form of complex aqueous mixtures. These mixtures contain the decay products of about 35 isotopes which are the nuclear fuel fission products, about 18 actinides and their daughter products as well as corrosion products of fuel cans and structural materials and chemical reagents added in the process of fuel reprocessing. The high-level radioactive waste management includes the liquid waste cooling which is necessary for the short and middle living isotope decay, separation of some most dangerous components from the waste mixture, waste solidification, their storage and disposal. The conclusion is drawn that the seccessful solution of the high-level radioactive waste management problem will permit to solve the problem of the fuel cycle radioactive waste management as a whole. The salt deposits, shales and clays are the most suitable for radioactive waste disposal [ru

A new class of medicament: radioactivity isotopes (1962); Une nouvelle classe de medicaments: les isotopes radioactifs (1962)

Energy Technology Data Exchange (ETDEWEB)

Cohen, Y. [Commissariat a l' Energie Atomique, Saclay (France). Centre d' Etudes Nucleaires

1962-07-01

Very many radioelement are used in medicine, either for diagnosis or as therapeutics. The development of medicine has entailed an increase in the number of application of radioactive isotopes. Firstly used in the form of simple inorganic molecules for diagnosis or as anticancer therapeutics, radioelements are now used for labelling organic molecules, allowing functional specific studies of any kind of nature. Their production is made difficult by their radio-active properties. Their pharmaceutical properties, determined by tests and controls, depend either from radiochemistry and from medicine. The author reminds, in this report, the methods for the preparation and analysis, and set out the medical application. (author) [French] De tres nombreux radioelements trouvent une application en medecine humaine, soit dans le diagnostic, soit en therapeutique. L'evolution de la medecine entraine un accroissement du champ d'application des isotopes radioactifs. D'abord utilises sous forme de molecules minerales simples, pour les diagnostics ou des therapeutiques anticancereuses, les radioelements sont maintenant introduits dans des molecules organiques qui permettent des etudes fonctionnelles specifiques de toute nature. Leur fabrication est compliquee par leurs proprietes radioactives. Leurs caracteristiques pharmaceutiques determinees par des essais et controles, sont liees d'une part a la radiochimie, d'autre part a la medecine. L'auteur rappelle, dans cet expose, les methodes de preparation et d'analyse et aborde les applications medicales. (auteur)

A new class of medicament: radioactivity isotopes (1962); Une nouvelle classe de medicaments: les isotopes radioactifs (1962)

Energy Technology Data Exchange (ETDEWEB)

Cohen, Y [Commissariat a l' Energie Atomique, Saclay (France). Centre d' Etudes Nucleaires

1962-07-01

Very many radioelement are used in medicine, either for diagnosis or as therapeutics. The development of medicine has entailed an increase in the number of application of radioactive isotopes. Firstly used in the form of simple inorganic molecules for diagnosis or as anticancer therapeutics, radioelements are now used for labelling organic molecules, allowing functional specific studies of any kind of nature. Their production is made difficult by their radio-active properties. Their pharmaceutical properties, determined by tests and controls, depend either from radiochemistry and from medicine. The author reminds, in this report, the methods for the preparation and analysis, and set out the medical application. (author) [French] De tres nombreux radioelements trouvent une application en medecine humaine, soit dans le diagnostic, soit en therapeutique. L'evolution de la medecine entraine un accroissement du champ d'application des isotopes radioactifs. D'abord utilises sous forme de molecules minerales simples, pour les diagnostics ou des therapeutiques anticancereuses, les radioelements sont maintenant introduits dans des molecules organiques qui permettent des etudes fonctionnelles specifiques de toute nature. Leur fabrication est compliquee par leurs proprietes radioactives. Leurs caracteristiques pharmaceutiques determinees par des essais et controles, sont liees d'une part a la radiochimie, d'autre part a la medecine. L'auteur rappelle, dans cet expose, les methodes de preparation et d'analyse et aborde les applications medicales. (auteur)

Status of radioactive ion beams at the HRIBF

CERN Document Server

Stracener, D W

2003-01-01

Radioactive Ion Beams (RIBs) at the Holifield Radioactive Ion Beam Facility (HRIBF) are produced using the isotope separation on-line technique and are subsequently accelerated up to a few MeV per nucleon for use in nuclear physics experiments. The first RIB experiments at the HRIBF were completed at the end of 1998 using sup 1 sup 7 F beams. Since then other proton-rich ion beams have been developed and a large number of neutron-rich ion beams are now available. The neutron-rich radioactive nuclei are produced via proton-induced fission of uranium in a low-density matrix of uranium carbide. Recently developed RIBs include sup 2 sup 5 Al from a silicon carbide target and isobarically pure beams of neutron-rich Ge, Sn, Br and I isotopes from a uranium carbide target.

Optical spectroscopy of laser-produced plasmas for standoff isotopic analysis

Energy Technology Data Exchange (ETDEWEB)

Harilal, Sivanandan S.; Brumfield, Brian E.; LaHaye, Nicole L.; Hartig, Kyle C.; Phillips, Mark C.

2018-04-20

This review article covers the present status of isotope detection through emission, absorption, and fluorescence spectroscopy of atoms and molecules in a laser-produced plasma formed from a solid sample. A description of the physics behind isotope shifts in atoms and molecules is presented, followed by the physics behind solid sampling of laser ablation plumes, optical methods for isotope measurements, the suitable physical conditions of laser-produced plasma plumes for isotopic analysis, and the current status. Finally, concluding remarks will be made on the existing gaps between previous works in the literature and suggestions for future work.

Fossil fuel produced radioactivities and their effect on foodchains

Energy Technology Data Exchange (ETDEWEB)

Okamoto, K [New South Wales Univ., Kensington (Australia). Dept. of Applied Mathematics

1980-10-01

The environmental impact of radioactivities produced from fossil fuel burning is not necessarily small compared with that of nuclear energy. The effect of these radioactivities on the foodchain through seafoods is discussed.

Secondary reactions as a tool to produce exotic nuclei

International Nuclear Information System (INIS)

Dufour, J.P.; Fleury, A.; Bimbot, R.

1980-01-01

The possibility of using secondary reactions as tool to produce new isotopes is considered. This question is renewed with the emergence of intense beams of energetic heavy ions in the range of 20 to 100 MeV/nucleon. Three different methods are considered. They involve either the 'in situ' production of a secondary radioactive target, which interacts with the primary beam, or the production of a radioactive secondary beam by an inverse fusion or a fragmentation process. Very heavy or very neutron deficient isotopes can be produced by these methods

Radioactivity. Centenary of radioactivity discovery

International Nuclear Information System (INIS)

Charpak, G.; Tubiana, M.; Bimbot, R.

1997-01-01

This small booklet was edited for the occasion of the exhibitions of the celebration of the centenary of radioactivity discovery which took place in various locations in France from 1996 to 1998. It recalls some basic knowledge concerning radioactivity and its applications: history of discovery, atoms and isotopes, radiations, measurement of ionizing radiations, natural and artificial radioactivity, isotope dating and labelling, radiotherapy, nuclear power and reactors, fission and fusion, nuclear wastes, dosimetry, effects and radioprotection. (J.S.)

The management of radioactive wastes from small producers

International Nuclear Information System (INIS)

1996-01-01

Medicine, research and industry generate various type of radioactive wastes which have to be managed by the ANDRA, the French agency for the management of radioactive wastes. This educative booklet explains the missions of the ANDRA with respect to these small producers: collection, selection, conditioning, control and storage of wastes. (J.S.)

Oxygen Isotope Composition of Nitrate Produced by Freshwater Nitrification

Science.gov (United States)

Boshers, D.; Granger, J.; Bohlke, J. K.

2016-12-01

Measurements of the naturally occurring nitrogen and oxygen stable isotope ratios of nitrate (NO3-), δ15N and δ18O, can be used to determine the source, dispersal, and fate of natural and contaminant NO3- in aquatic environments. To this end, it is necessary to know the extent to which NO3- isotopologues are modified by biological reactions, as heavy and light isotopes have different reaction rates. The purpose of this study was to determine the influence of the δ18O of ambient water on the isotope composition of NO3- produced during nitrification, the biological oxidation of ammonium (NH4+) to nitrite (NO2-) and then NO3-, which is poorly constrained in freshwater systems. To determine the δ18O of NO3- produced by nitrification in freshwater, we collected water from a stream in New England, which we amended with NH4+ and with increments of 18O-enriched water, to monitor the isotope composition of NO3- produced by a natural consortium of nitrifiers. Added NH4+ was completely oxidized to NO3- over 26 days. The final δ18O of nitrified NO3- revealed sensitivity to the δ18O of water mediated by (a) isotopic equilibration between water and NO2- and (b) kinetic isotope fractionation during O-atom incorporation from water into NO2- and NO3-. Our results concur with nitrifying culture experiments that have demonstrated analogous sensitivity of the δ18O of nitrified NO3- to equilibrium and kinetic O isotope effects (Buchwald et al. 2012), as well as show that these dynamics need to be considered to interpret NO3- isotope distribution in freshwater environments.

Expeditious syntheses of stable and radioactive isotope-labeled anticonvulsant agent, JNJ-26990990, and its metabolites.

Science.gov (United States)

Lin, Ronghui; Weaner, Larry E; Hoerr, David C; Salter, Rhys; Gong, Yong

2013-01-01

Syntheses of stable and radioactive isotope-labeled anticonvulsant agent, JNJ-26990990, that is, N-(benzo[b]thien-3-ylmethyl)-sulfamide and its metabolites are described. [(13)C(15)N]Benzo[b]thiophene-3-carbonitrile was first prepared by coupling of 3-bromo-benzo[b]thiophene with [(13)C(15)N]-copper cyanide. The resultant [(13)C(15)N]benzo[b]thiophene-3-carbonitrile was reduced with lithium aluminum deuteride to give [(13)CD2(15)N]benzo[b]thiophen-3-yl-methylamine; which was then coupled with sulfamide to afford [(13)CD2(15)N]-N-(benzo[b]thien-3-ylmethyl)-sulfamide, the stable isotope-labeled compound with four stable isotope atoms. Direct oxidation of [(13)CD2(15)N]-N-(benzo[b]thien-3-ylmethyl)-sulfamide with hydrogen peroxide and peracetic acid gave the stable isotope-labeled sulfoxide and sulfone metabolites. On the other hand, radioactive (14)C-labeled N-(benzo[b]thien-3-ylmethyl)-sulfamide was prepared conveniently by sequential coupling of 3-bromo-benzo[b]thiophene with [(14)C]-copper cyanide, reduction of the carbonitrile to carboxaldehyde, and reductive amination with sulfamide. Copyright © 2013 John Wiley & Sons, Ltd.

Natural radioactivity in food chains

Energy Technology Data Exchange (ETDEWEB)

Binnerts, W

1989-03-01

A number of longliving and still being produced radioactive isotopes produces well measurable and not to be neglected radiation, by which, via the food chains, plant, animal and man receives a socalled natural radiation dose. Six of the most important isotopes are discussed here. The radioisotopes /sup 14/C and /sup 40/K form part of the most live-necessary elements; they pass without strong enrichment and discrimination through the food chains and form a practically constant part of the living organism. Yet by excessive fertilizing a rather higher content of potassium than necessary is present in plants. Also a higher radiation dose arises from exessive uptake of food. The isotopes of uranium /sup 238/U and radium, /sup 226/Ra, discussed here, occur everywhere in the soil, but locally in very high amounts. They migrate for a very small part into plant and animal, sometimes occur in vegetable food as part of soil particles. Other important isotopes of the uranium families are radioactive lead, /sup 21/0Pb, and polonium, /sup 210/Po, which can be dispersed to a much greater amount than the other isotopes: in the form of the gaseous intermediate product radon, here the isotope /sup 222/Rn. /sup 210/Pb and /sup 210/Po are finally deposited upon plants and other food products. In the hydrosphere /sup 210/Po can be enriched in the food chain from plankton to fish. (author). 35 refs.; 2 figs.; 3 tabs.

Natural radioactivity in food chains

International Nuclear Information System (INIS)

Binnerts, W.

1989-01-01

A number of longliving and still being produced radioactive isotopes produces well measurable and not to be neglected radiation, by which, via the food chains, plant, animal and man receives a socalled natural radiation dose. Six of the most important isotopes are discussed here. The radioisotopes 14 C and 40 K form part of the most live-necessary elements; they pass without strong enrichment and discrimination through the food chains and form a practically constant part of the living organism. Yet by excessive fertilizing a rather higher content of potassium than necessary is present in plants. Also a higher radiation dose arises from exessive uptake of food. The isotopes of uranium 238 U and radium, 226 Ra, discussed here, occur everywhere in the soil, but locally in very high amounts. They migrate for a very small part into plant and animal, sometimes occur in vegetable food as part of soil particles. Other important isotopes of the uranium families are radioactive lead, 21 0Pb, and polonium, 210 Po, which can be dispersed to a much greater amount than the other isotopes: in the form of the gaseous intermediate product radon, here the isotope 222 Rn. 210 Pb and 210 Po are finally deposited upon plants and other food products. In the hydrosphere 210 Po can be enriched in the food chain from plankton to fish. (author). 35 refs.; 2 figs.; 3 tabs

Uranium isotopes as radioactive pollutants in groundwaters of the Morro do Ferro thorium deposit, Brazil

International Nuclear Information System (INIS)

Bonotto, D.M.

1991-01-01

Groundwater and surface water samples were collected at Morro do Ferro, a thorium and rare earth deposit located on the Pocos de Caldas Plateau, Minas Gerais State, Brazil, to evaluate if the mechanisms related to the migration of 238 U and 234 U isotopes can generate concentrations greater than the gross-alpha activity contaminant limit. The 238 U content range was 0.003-0.24 pCi/1 and the 234 U content range was 0.004-0.25 pCi/1, showing that the studied hydrologic environment doesn't indicate pollution by radioactivity due to these nuclides. However, 226 Ra and 228 Ra isotopes can be considered as radioactive pollutants in groundwaters but not in surface waters of the Morro do Ferro. (author)

Optical spectroscopy of laser-produced plasmas for standoff isotopic analysis

Science.gov (United States)

Harilal, S. S.; Brumfield, B. E.; LaHaye, N. L.; Hartig, K. C.; Phillips, M. C.

2018-06-01

Rapid, in-field, and non-contact isotopic analysis of solid materials is extremely important to a large number of applications, such as nuclear nonproliferation monitoring and forensics, geochemistry, archaeology, and biochemistry. Presently, isotopic measurements for these and many other fields are performed in laboratory settings. Rapid, in-field, and non-contact isotopic analysis of solid material is possible with optical spectroscopy tools when combined with laser ablation. Laser ablation generates a transient vapor of any solid material when a powerful laser interacts with a sample of interest. Analysis of atoms, ions, and molecules in a laser-produced plasma using optical spectroscopy tools can provide isotopic information with the advantages of real-time analysis, standoff capability, and no sample preparation requirement. Both emission and absorption spectroscopy methods can be used for isotopic analysis of solid materials. However, applying optical spectroscopy to the measurement of isotope ratios from solid materials presents numerous challenges. Isotope shifts arise primarily due to variation in nuclear charge distribution caused by different numbers of neutrons, but the small proportional nuclear mass differences between nuclei of various isotopes lead to correspondingly small differences in optical transition wavelengths. Along with this, various line broadening mechanisms in laser-produced plasmas and instrumental broadening generated by the detection system are technical challenges frequently encountered with emission-based optical diagnostics. These challenges can be overcome by measuring the isotope shifts associated with the vibronic emission bands from molecules or by using the techniques of laser-based absorption/fluorescence spectroscopy to marginalize the effect of instrumental broadening. Absorption and fluorescence spectroscopy probe the ground state atoms existing in the plasma when it is cooler, which inherently provides narrower

Hyperaccumulation of radioactive isotopes by marine algae

International Nuclear Information System (INIS)

Ishii, Toshiaki; Hirano, Shigeki; Watabe, Teruhisa

2003-01-01

Hyperaccumlators are effective indicator organisms for monitoring marine pollution by heavy metals and artificial radionuclides. We found a green algae, Bryopsis maxima that hyperaccumulate a stable and radioactive isotopes such as Sr-90, Tc-99, Ba-138, Re-187, and Ra-226. B. maxima showed high concentration factors for heavy alkali earth metals like Ba and Ra, compared with other marine algae in Japan. Furthermore, this species had the highest concentrations for Tc-99 and Re-187. The accumulation and excretion patterns of Sr-85 and Tc-95m were examined by tracer experiments. The chemical states of Sr and Re in living B. maxima were analyzed by HPLC-ICP/MS, LC/MS, and X-ray absorption fine structure analysis using synchrotron radiation. (author)

The natural radioactivity of the biosphere

Energy Technology Data Exchange (ETDEWEB)

Pertsov, L A

1967-07-01

Of the approximately 1200 isotopes presently known more than 900 are radioactive. The nuclei of these isotopes are unstable and decay spontaneously emitting ionizing gamma-, alpha- or beta-radiation. The overwhelming majority of known radioactive isotopes have been obtained artificially; only a few are natural. Numerous investigations have shown that many of the natural radioactive isotopes can be grouped into three radioactive families. Each such family is characterized by the existence of one long-lived isotope - the family parent, one gaseous isotope of radon, intermediate radioactive decay products and final stable isotopes of atomic weights 206, 207 and 208. No such generic relationship has been established among the remaining natural radioactive isotopes. The purpose of the book, in contrast to some recent review works, is to present, in addition to a summary of reference data characterizing the radioactivity levels of various components of the biosphere, a description of those phenomena and regularities which will apparently make it possible to understand more completely the basic dynamics of the natural radioactivity of the biosphere and, consequently, contribute to a more correct interpretation of radiation-hygiene in each specific case.

The natural radioactivity of the biosphere

International Nuclear Information System (INIS)

Pertsov, L.A.

1967-01-01

Of the approximately 1200 isotopes presently known more than 900 are radioactive. The nuclei of these isotopes are unstable and decay spontaneously emitting ionizing gamma-, alpha- or beta-radiation. The overwhelming majority of known radioactive isotopes have been obtained artificially; only a few are natural. Numerous investigations have shown that many of the natural radioactive isotopes can be grouped into three radioactive families. Each such family is characterized by the existence of one long-lived isotope - the family parent, one gaseous isotope of radon, intermediate radioactive decay products and final stable isotopes of atomic weights 206, 207 and 208. No such generic relationship has been established among the remaining natural radioactive isotopes. The purpose of the book, in contrast to some recent review works, is to present, in addition to a summary of reference data characterizing the radioactivity levels of various components of the biosphere, a description of those phenomena and regularities which will apparently make it possible to understand more completely the basic dynamics of the natural radioactivity of the biosphere and, consequently, contribute to a more correct interpretation of radiation-hygiene in each specific case

Production of exotic beams by separation of online isotope

International Nuclear Information System (INIS)

Hosni, Faouzi; Farah, K.

2013-01-01

The studies in physics, concerned until now, approximately two thousand five hundred radioactive nuclide. These nuclides with 263 stable nucleus constitute the current nuclear field. This field is far from being complete because there are more than three thousand radioactive isotopes to be discovered. Materials and Methods: To reach these radio-isotopes there are two complementary methods which are the on-line separation (ISOL) and the fragmentation in times of flight. The latter has the advantage to allow the study of the elements of very short period (lower than 10-3 s). It supplies beams having a big dispersal in energy and in angle. In the case of the separation of on-line isotope, a target is run to produce the radioactive atoms. This allows producing beams much more intense than the fragmentation in times of flight. To obtain radioactive beams in the required intensities or for the research or medical applications, it is essential to end in thick targets or the products of reaction can go out as fast as possible. That is to realize targets which can maintain a porous and sluggish structure counterpart in the produced elements. This is one of the main technological challenges to be solved. The works concerning this domain will be presented as well as the got advantage if the nuclear reactions are led by protons reaching 30 MeV of energy. (Author)

Radioactive ion beam facilities at INFN LNS

International Nuclear Information System (INIS)

Rifuggiato, D; Calabretta, L; Celona, L; Chines, F; Cosentino, L; Cuttone, G; Finocchiaro, P; Pappalardo, A; Re, M; Rovelli, A

2011-01-01

Radioactive ion beams are produced at INFN- Laboratori Nazionali del Sud (LNS) by means of the two operating accelerators, the Tandem and the Superconducting Cyclotron (CS), originally designed to accelerate stable beams. Both the ISOL (Isotope Separation On Line) and the IFF (In-Flight Fragmentation) methods are exploited to produce RIBs in two different ways at different energies: in the first case, the Cyclotron is the primary accelerator and the Tandem accelerates the secondary beams, while in the second case radioactive fragments are produced by the Cyclotron beam in a thin target with energies comparable to the primary beam energy. The ISOL facility is named EXCYT (Exotics at the Cyclotron and Tandem) and was commissioned in 2006, when the first radioactive beam ( 8 Li) has been produced. The IFF installation is named FRIBs (in Flight Radioactive Ion Beams), and it has started to produce radioactive beams in 2001, placing a thin target in the extraction beam line of the Cyclotron. The development of both facilities to produce and accelerate radioactive ion beams at LNS, is briefly described, with some details on the future prospects that are presently under consideration or realization.

Calculation of radioactive decay chains produced by neutron irradiation

International Nuclear Information System (INIS)

Ponti, C.

1984-01-01

The calculation of the decay chains of radioactive isotopes may be solved by different computer codes that apply similar numerical methods. Analytical forms of solution of this problem are known since a long time, but their implementation has always been hindered by the possible occurrence of large numerical errors or by the need, to avoid them, of very high numerical precision. In this paper the reason of these difficulties has been pointed out and solved. In particular a new family of mathematical identities has been found

BEARS: Radioactive ion beams at LBNL

International Nuclear Information System (INIS)

Powell, J.; Guo, F.Q.; Haustein, P.E.

1998-01-01

BEARS (Berkeley Experiments with Accelerated Radioactive Species) is an initiative to develop a radioactive ion-beam capability at Lawrence Berkeley National Laboratory. The aim is to produce isotopes at an existing medical cyclotron and to accelerate them at the 88 inch Cyclotron. To overcome the 300-meter physical separation of these two accelerators, a carrier-gas transport system will be used. At the terminus of the capillary, the carrier gas will be separated and the isotopes will be injected into the 88 inch Cyclotron's Electron Cyclotron Resonance (ECR) ion source. The first radioactive beams to be developed will include 20-min 11 C and 70-sec 14 O, produced by (p,n) and (p,α) reactions on low-Z targets. A test program is currently being conducted at the 88 inch Cyclotron to develop the parts of the BEARS system. Preliminary results of these tests lead to projections of initial 11 C beams of up to 2.5 x 10 7 ions/sec and 14 O beams of 3 x 10 5 ions/sec

Investigation of produced waters radioactivity of oil and gas deposits in the Dnieper-Donets province

Directory of Open Access Journals (Sweden)

Plyatsuk L. D.

2017-12-01

Full Text Available The process of radioactive pollution of produced waters, oilfield equipment, oil-contaminated soils and sludge is widely spread and differs within the various oil and gas regions. Formation waters contained radioactive element isotopes become the significant source and cause of elevated level of equivalent dose power and as a consequence, an increase in the incidence among the population. The author's idea is formulation of specific recommendations on the decontamination of the investigated objects by conducting the necessary appropriate experimental studies. The purpose of the article is to determine the content of radionuclides, γ- and α-emitters in technogenic objects of Bugruvate oil and gas fields, and to reveal the relationship with the features of mineralogical composition, geological structure and technological process. The γ-spectrometric analysis was used to determine the radionuclide composition of the natural radiators of the 238U (226Ra, 214Pо, 214Bi and 232Th (228Ac, 212Pb, 212Вi series in samples of technological sludge, oil, individual soil samples and water. The content of radionuclides of α-emitters was determined using separate radiochemical techniques. It was investigated that the radioactivity of the formation water is mainly determined by 226Ra and 228Ra and the products of their decay.

Behaviour of radioactive and stable isotopes of calcium in the soil-solution-plant system at different soil humidity

International Nuclear Information System (INIS)

Karavaeva, E.N.; Molchanova, I.V.

1976-01-01

The results of experiments performed to study the behaviour of radioactive and stable isotopes of Ca in soil - solution - plant system at different soil moistening are given. The experiments have been conducted in culture pans with two soils: soddy-meadow and soddy-podzolic differing in a number of physico-chemical properties. The solution of radioactive Ca( 45 CaCl 2 ) has been applied to soddy-meadow soil at the rate of 0.2 μcurie/kg, and to soddy-podzolic soil - at the rate of 0.1 μcurie/kg. The distribution and accumulation coefficients are estimated by the ratio to the total content of stable Ca and 45 Ca in soil. A direct relationship between distribution coefficients and the rate of soil moistening is observed. It has been established that 45 Ca and the natural stable isotopes of Ca applied to the soil differ in the type of distribution in soil - soil solution system and in accumulation by plants. However, a great similarity has been observed in behaviour of radioactive and stable isotopes of Ca depending on soil moistening

Hyperfine spectra of the radioactive isotopes 81Kr and 85Kr

International Nuclear Information System (INIS)

Cannon, B.D.

1993-01-01

Isotope shifts and hyperfine constants are reported for the radioactive isotopes 81 Kr and 85 Kr and the stable isotope 83 Kr. The previously unreported nuclear moments of 81 Kr were determined to be μ I =-0.909(4) nuclear magneton and Q=+0.630(13) b from the hyperfine constants. This work increases the number of transitions for which 85 Kr hyperfine constants and isotope shifts have been measured from 1 to 4. The hyperfine anomaly for krypton reported in the previous measurement of 85 Kr hyperfine constants [H. Gerhardt et al., Hyperfine Interact. 9, 175 (1981)] is not supported by this work. The isotope shifts and hyperfine constants of 83 Kr measured in this work are in excellent agreement with previous work. Saturation spectroscopy was used to study transitions from krypton's metastable 1s 5 state to the 2p 9 , 2p 7 , and 2p 6 states. In saturation spectra, different line shapes were observed for the even- and odd-mass krypton isotopes. This even- versus odd-line-mass shape difference can be explained using the large cross section that has been reported for collisional transfer of the 1s 5 state excitation between krypton atoms. Two-color two-photon laser-induced fluorescence was used to measure the hyperfine spectra of the 1s 5- 4d 4 ' transition using the 2p 9 state as the intermediate state. This technique proved to be more sensitive than saturation spectroscopy

Fishing for isotopes in the Brookhaven Lab Isotope Producer (BLIP) cooling water

Energy Technology Data Exchange (ETDEWEB)

Fitzsimmons, Jonathan [Brookhaven National Lab. (BNL), Upton, NY (United States). Collider Accelerator Dept.

2016-04-29

Be-7 has been used in environmental studies; the isotope is produced during BLIP irradiations and accumulates in the 320 gallons of cooling water. Be-7 has a 53.24 day half-life, so the optimal production/purification time is at the end of the BLIP run season. To purify Be-7 fifteen to twenty gallons of BLIP cooling water are removed and pumped through ion exchange columns that retain Be-7. This labor intensive approach captures ~15 mCi of Be-7, but the solution requires further purification. The method can lead to increased radiation exposure to staff. The ideal way to capture isotopes from large volumes is to reach in to the solution and selectively pull out the desired isotope. It is a lot like fishing.

The cobalt radioactive isotopes in environment

International Nuclear Information System (INIS)

2007-01-01

For the year 1993 the total activity released in cobalt is 69 GBq for the whole of nuclear power plants. The part of activity in cobalt for La Hague in 1993 is 8 GBq of 58 Co and 2 GBq of 60 Co. The radioactive isotopes released by nuclear power plants or the reprocessing plant of La Hague under liquid effluents are shared by half between 58 Co and 60 Co. The exposure to sealed sources is the most important risk for the cobalt. The risk of acute exposure can associate a local irradiation of several decades of grays inducing a radiological burns, deep burn to treat in surgery by resection or graft even amputation. A global irradiation of organism for several grays induces an acute irradiation syndrome, often serious. At long term the stochastic effects are represented by leukemia and radio-induced cancers. The increase of probability of their occurrence is 1% by sievert. We must remind that the natural spontaneous probability is 25%. (N.C.)

Radiography of light alloy castings using radioactive isotopes

International Nuclear Information System (INIS)

Lakshminarayana, A.R.; Ramamurthy, D.

1977-01-01

One of the most important causes for setback of nation's economy is loss of productive elements as a result of avoidable accidents. Particularly in a complicated field such as aircraft production, failure of a single part may cause the loss of men, money and materials which are all productive elements. To reduce such a loss, to increase productivity and to earn customer confidence, it is absolutely necessary to find out tools for quality assurance of defect prone castings. Radioactive isotopes can judiciously be employed inspite of its lower contrast, provided the radiographer understands : (1) the various types of defects characteristics of each alloy and (2) the limitations and possibilities of detecting such defects by this method. (author)

Isotopes as Tracers of the Hawaiian Coffee-Producing Regions

Science.gov (United States)

2011-01-01

Green coffee bean isotopes have been used to trace the effects of different climatic and geological characteristics associated with the Hawaii islands. Isotope ratio mass spectrometry (IRMS) and inductively coupled plasma mass spectrometry ((MC)-ICP-SFMS and ICP-QMS) were applied to determine the isotopic composition of carbon (δ13C), nitrogen (δ15N), sulfur (δ34S), and oxygen (δ18O), the isotope abundance of strontium (87Sr/86Sr), and the concentrations of 30 different elements in 47 green coffees. The coffees were produced in five Hawaii regions: Hawaii, Kauai, Maui, Molokai, and Oahu. Results indicate that coffee plant seed isotopes reflect interactions between the coffee plant and the local environment. Accordingly, the obtained analytical fingerprinting could be used to discriminate between the different Hawaii regions studied. PMID:21838232

Treatment of radioactive effluents at the Boris Kidric Institute; Postupak sa radioaktivnim elementima u Institutu Boris Kidric

Energy Technology Data Exchange (ETDEWEB)

Bojovic, P; Drobnik, S; Popara, D [Institute of Nuclear Sciences Vinca, Beograd (Serbia and Montenegro)

1964-10-15

The paper describes the origin, composition and activity of radioactive effluents at the Boris Kidric Institute, their collection at the places or origin, transport to the place of disposal and treatment of some smaller quantities. Special attention has been paid to effluents with short-lived isotopes produced in the Laboratory for radioactive isotope production (author)

Nuclear charge radius measurements of radioactive beryllium isotopes

CERN Multimedia

2002-01-01

We propose to measure the nuclear charge radii of the beryllium isotopes $^{7,9,10}$Be and the one-neutron halo isotope $^{11}$Be using laser spectroscopy of trapped ions. Ions produced at ISOLDE and ionized with the laser ion source will be cooled and bunched in the radio-frequency buncher of the ISOLTRAP experiment and then transferred into a specially designed Paul trap. Here, they will be cooled to temperatures in the mK range employing sympathetic and direct laser cooling. Precision laser spectroscopy of the isotope shift on the cooled ensemble in combination with accurate atomic structure calculations will provide nuclear charge radii with a precision of better than 3%. This will be the first model-independent determination of a one-neutron halo nuclear charge radius.

The Safe Transportation of Radioactive Materials

International Nuclear Information System (INIS)

Megrahi, Abdulhafeed; Abu-Ali, Giuma; Enhaba; Ahmed

2008-01-01

In this paper, we present the essential conditions that should be required for transporting the radioactive materials. We demonstrate the procedure for transporting the radioactive iodine-131 from the Centre of Renewable Energies and Desalination of Water in Tajoura, Libya to Tripoli Medical Center. The safe measures were taken during the process of the transportation of the isotope produced in the centre including dosimetry analysis and the thickness of the container. (author)

IUPAC Periodic Table of Isotopes for the Educational Community

International Nuclear Information System (INIS)

Holden, N.E.; Coplen, T.B.

2012-01-01

John Dalton first proposed the concept of atomic weights of the elements in the first decade of the nineteenth century. These atomic weights of the chemical elements were thought of as constants of nature, similar to the speed of light. Dmitri Mendeleev arranged the atomic weights of the elements in ascending order of value and used the systematic variation of their chemical properties to produce his Periodic Table of the Elements in 1869. Measurement of atomic weight values became an important chemical activity for a century and a half. Theodore Richards received a Noble Prize for his work in this area. In 1913, Fredrick Soddy found a species of radium, which had an atomic weight value of 228, compared to the familiar radium gas value of 226. Soddy coined the term 'isotope' (Greek for 'in the same place') to account for this second atomic weight value in the radium position of the Periodic Table. Both of these isotopes of radium are radioactive. Radioactive isotopes are energetically unstable and will decay (disintegrate) over time. The time it takes for one half of a sample of a given radioactive isotope to decay is the half-life of that isotope. In addition to having different atomic weight values, radium-226 and radium-228 also have different half-life values. Around the same time as Soddy's work, J.J. Thomson (discoverer of the electron) identified two stable (non-radioactive) isotopes of the same element, neon. Over the next 40 years, the majority of the known chemical elements were found to have two or more stable (or long-lived radioactive isotopes that contribute significantly to the determination of the atomic weights of the elements).

Uses of Radioactive Isotopes in Industry; Aplicacion es de los isotopos radiactivos en la industria

Energy Technology Data Exchange (ETDEWEB)

Plata, A; Val Cob, M del; Gamboa, J M

1962-07-01

The present report contains a list of some of the most important problems in industry that have been approached so far by the use of radioactive isotopes. The list has been compiled trough the experience gained by the authors in revising for several years the most important scientific journal and other sources of information on this subject. The classification of industries has been done in an arbitrary way, choosing those isotope uses that have reached a higher degree of development. (Author)

From the discovery of radioactivity to the production of radioactive beams

International Nuclear Information System (INIS)

Bimbot, R.

1999-01-01

The evolution of the projectiles used to explore the nucleus influenced strongly the development of Nuclear Physics. The alpha particles from radioactivity were the projectiles mostly used up to the second world war. This period was marked by fundamental discoveries, as those of artificial radioactivity and of fission. From the 1930's to 1070, light accelerated particles (electrons, protons, deuterons, isotopes of helium) became universally used. A third period began in the 1960's with the emergence of heavy ion accelerators, the use of which led to a true revolution in the study of nuclear matter. Finally, the fourth period started in 1985 when the first secondary beams of radioactive nuclei were produced, and opened new ways in physics. (authors)

Set of devices for producing radioactive 60Co-sources

International Nuclear Information System (INIS)

Eichhorn, P.; Tobisch, F.

1982-01-01

A set of devices for producing radioactive 60 Co-sources was developed. A single source has a radioactivity of 445x10 10 GBq. It consists of a double envelope of stainless steel filled with a mixture of small pieces of cobalt and stainless steel wire. The diameter of a source is 11 mm; the length 80 mm. Cobalt wires of different radioactivity with a length of about 110 mm and 0,8 mm diameter are the raw material. The set is located in a hot cell. Construction, functions and operation of the set are described in detail. (author)

Radioactive cesium isotope ratios as a tool for determining dispersal and re-dispersal mechanisms downwind from the Nevada Nuclear Security Site.

Science.gov (United States)

Snyder, Darin C; Delmore, James E; Tranter, Troy; Mann, Nick R; Abbott, Michael L; Olson, John E

2012-08-01

Fractionation of the two longer-lived radioactive cesium isotopes ((135)Cs and (137)Cs) produced by above ground nuclear tests have been measured and used to clarify the dispersal mechanisms of cesium deposited in the area between the Nevada Nuclear Security Site and Lake Mead in the southwestern United States. Fractionation of these isotopes is due to the 135-decay chain requiring several days to completely decay to (135)Cs, and the 137-decay chain less than one hour decay to (137)Cs. Since the Cs precursors are gases, iodine and xenon, the (135)Cs plume was deposited farther downwind than the (137)Cs plume. Sediment core samples were obtained from the Las Vegas arm of Lake Mead, sub-sampled and analyzed for (135)Cs/(137)Cs ratios by thermal ionization mass spectrometry. The layers proved to have nearly identical highly fractionated isotope ratios. This information is consistent with a model where the cesium was initially deposited onto the land area draining into Lake Mead and the composite from all of the above ground shots subsequently washed onto Lake Mead by high intensity rain and wind storms producing a layering of Cs activity, where each layer is a portion of the composite. Copyright © 2012 Elsevier Ltd. All rights reserved.

Study on Method of Asphalt Density Measurement Using Low Level Radioactive Isotope

International Nuclear Information System (INIS)

Chung, Jin-young; Kim, Jung-hoon; Whang, Joo-ho

2008-01-01

The fundamental cause of damage to road pavement is insufficient management of asphalt density during construction. Currently, asphalt density in Korea is measured in a laboratory by extracting a core sample after construction. This method delays the overall time of measurement and therefore it is difficult to achieve real-time density management. Using a radioactive isotope for measuring asphalt density during construction reduces measuring time thus enabling realtime measurement. Also, it is provided reliable density measurement to achieve effective density management at work sites. However, existing radiological equipment has not been widely used because of management restrictions and regulations due to the high radiation dose. In this study, we employed a non-destructive method for density measurement. Density is measured by using a portable gamma-ray backscatter device having a radioactivity emission of 100 μCi or less (notice No. 2002-23, Ministry of Science and Technology, standards on radiation protection, etc.), a sealed radioactive source subject to declaration

Isotopic marking and tracers

International Nuclear Information System (INIS)

Morel, F.

1997-01-01

The use of radioactive isotopes as tracers in biology has been developed thanks to the economic generation of the required isotopes in accelerators and nuclear reactors, and to the multiple applications of tracers in the life domain; the most usual isotopes employed in biology are carbon, hydrogen, phosphorus and sulfur isotopes, because these elements are present in most of organic molecules. Most of the life science knowledge appears to be dependent to the extensive use of nuclear tools and radioactive tracers; the example of the utilization of radioactive phosphorus marked ATP to study the multiple reactions with proteins, nucleic acids, etc., is given

IUPAC Periodic Table of Isotopes for the Educational Community

Energy Technology Data Exchange (ETDEWEB)

Holden N. E.; Holden,N.E.; Coplen,T.B.

2012-07-15

John Dalton first proposed the concept of atomic weights of the elements in the first decade of the nineteenth century. These atomic weights of the chemical elements were thought of as constants of nature, similar to the speed of light. Dmitri Mendeleev arranged the atomic weights of the elements in ascending order of value and used the systematic variation of their chemical properties to produce his Periodic Table of the Elements in 1869. Measurement of atomic weight values became an important chemical activity for a century and a half. Theodore Richards received a Noble Prize for his work in this area. In 1913, Fredrick Soddy found a species of radium, which had an atomic weight value of 228, compared to the familiar radium gas value of 226. Soddy coined the term 'isotope' (Greek for 'in the same place') to account for this second atomic weight value in the radium position of the Periodic Table. Both of these isotopes of radium are radioactive. Radioactive isotopes are energetically unstable and will decay (disintegrate) over time. The time it takes for one half of a sample of a given radioactive isotope to decay is the half-life of that isotope. In addition to having different atomic weight values, radium-226 and radium-228 also have different half-life values. Around the same time as Soddy's work, J.J. Thomson (discoverer of the electron) identified two stable (non-radioactive) isotopes of the same element, neon. Over the next 40 years, the majority of the known chemical elements were found to have two or more stable (or long-lived radioactive isotopes that contribute significantly to the determination of the atomic weights of the elements).

Problems in producing nuclear reactor for medical isotopes and the Global Crisis of molybdenum supply; Problemas en la produccion en reactores nucleares de isotopos con fines medicos y la crisis mundial de suministro de molibdeno ({sup 9}9Mo)

Energy Technology Data Exchange (ETDEWEB)

Zubiarrain, A.

2011-07-01

Nuclear medicine uses drugs that incorporate a radioactive isotope radiopharmaceuticals. Every year are performed, worldwide, 35 million nuclear medicine procedures, of which 80% are done with radiopharmaceuticals containing the isotope, molybdenum-99, produced in nuclear reactors. In recent years, there have been several supply crisis of molybdenum-99, which have hampered diagnostic procedure with technitium-99m. (Author)

Electroplating method for producing ultralow-mass fissionable deposits

International Nuclear Information System (INIS)

Ruddy, F.H.

1989-01-01

A method for producing ultralow-mass fissionable deposits for nuclear reactor dosimetry is described, including the steps of holding a radioactive parent until the radioactive parent reaches secular equilibrium with a daughter isotope, chemically separating the daughter from the parent, electroplating the daughter on a suitable substrate, and holding the electroplated daughter until the daughter decays to the fissionable deposit

New Applications of Cosmogenic Radioactive Isotopes to Study Water Travel Times

Science.gov (United States)

Visser, A.; Thaw, M.; Deinhart, A.; Bibby, R. K.; Esser, B.

2017-12-01

The travel time of water moving through a landscape influences nutrient dynamics and biogeochemical cycles. Constraining water travel times helps to understand the functioning of the critical zone. Water travel times cannot be observed directly but can be constrained by measurements of cosmogenic radioactive isotopes. We studied a small (4.6 km2) subalpine (1660-2117 m) catchment in a Mediterranean climate (8 °C, 1200 mm/yr) in the California Sierra Nevada to assess subsurface water storage dynamics and investigate flow paths and flow velocities. We analyzed a combination of three cosmogenic radioactive isotopes with half-lives varying from 87 days (sulfur-35), 2.6 years (sodium-22) to 12.3 years (tritium) in precipitation and stream samples. Water stable isotopes and solute chemistry aided the interpretation of the cosmogenic isotopes. Tritium samples (1L) are analyzed by noble gas mass spectrometry after helium-3 accumulation. Samples for sulfur-35 and sodium-22 are collected by processing 20-1000 L of water through an anion and cation exchange column in-situ. Sulfur-35 is analyzed by liquid scintillation counting after chemical purification and precipitation. Sodium-22 is analyzed by gamma counting after eluting the cations into a 4L Marinelli beaker. Monthly collected precipitation samples show variability of deposition rate for tritium and sulfur-35. Sodium-22 levels in cumulative yearly precipitation samples are consistent with recent studies in the US and Japan. The observed variability of deposition rates complicates direct use as decaying age tracers. The level and variability of tritium in monthly stream samples indicate a mean residence time on the order of 10 years and only small contributions of younger water during high flow conditions. Sulfur-35 and sodium-22 concentrations were critically interpreted considering possible uptake by vegetation and cation exchange. Detections of sodium-22 confirm a small fraction of younger (water. Low concentrations

The use of natural radioactive Isotopes in the determination of pollution sources of AL-Kabir AL-Shimali river

International Nuclear Information System (INIS)

Al-Masri, M. S.; Shwiekani, R.; Mamish, S.

2012-01-01

In the present research, variations of concentration levels of some natural radioactive isotopes (226 Ra, 210 Po,210 Pb, U and Th isotopes) and some trace elements (Cu, Zn, Pb, Cd) in water and sediments of AL-Kabir AL-Shimali river during the period of 2009-2010 have been studied. The samples were collected along the river from the asphalt factory to the end of the mouth of the river in the Mediterranean Sea. Results showed that concentrations of natural radioactive isotopes have been increased slightly in water and sediments of the river after the asphalt factory and after the factories area, while the concentrations of Rn in the river's water were low along the river except the waters of October 16, Lake Dam that reached a value of 341 mBq/l. These high concentrations in water and sediments of the AL-Kabir AL-Shimali River were due to discharges from the asphalt factory and other factories known to contain natural radioactive isotopes, indicating the possibility of using these isotopes in the determination of pollution sources of AL-Kabir AL-Shimali River. However, the measured concentrations are relatively low compared to the values reported in the world due to river water flow that dilute concentrations of these elements. On the other hand, measurements of trace elements (Cu,Zn,Pb,Cd) showed low concentrations in the waters of the river, with some increases in the concentrations in river sediments after the asphalt factory and the factories area , indicating the contribution of the factories outlets in this increase. The results were compared with the results of previous studies conducted on the Euphrates and the Orontes, where the comparison showed lower values in the AL-Kabir AL-Shimali river environment. (author)

The use of natural radioactive isotopes in the determination of pollution sources of Al-Kabir Al-Shimali river

International Nuclear Information System (INIS)

ALmasri, M.; Shweikani, R.; Mamish, S.; Al-Haleem, M.A.; Al-Shamali, K.; Jerby, B.

2010-10-01

In the present research, variations of concentration levels of some natural radioactive isotopes ( 226 Ra, 210 Po, 210 Pb, U and Th isotopes) and some trace elements (Cu, Zn, Pb, Cd) in water and sediments of Al-Kabir Al-Shimali river during the period of 2009-2010 have been studied. The samples were collected along the river from the asphalt factory to the end of the mouth of the river in the Mediterranean Sea. Results showed that concentrations of natural radioactive isotopes have been increased slightly in water and sediments of the river after the asphalt factory and after the factories area, while the concentrations of Rn in the river's water were low along the river except the waters of October 16, Lake Dam that reached a value of 341mBq/l. These high concentrations in water and sediments of the Al-Kabir Al-Shimali River were due to discharges from the asphalt factory and other factories known to contain natural radioactive isotopes, indicating the possibility of using these isotopes in the determination of pollution sources of Al-Kabir Al-Shimali River. However, the measured concentrations are relatively low compared to the values reported in the world due to river water flow that dilute concentrations of these elements. On the other hand, measurements of trace elements (Cu,Zn,Pb,Cd) showed low concentrations in the waters of the river, with some increases in the concentrations in river sediments after the asphalt factory and the factories area , indicating the contribution of the factories outlets in this increase. The results were compared with the results of previous studies conducted on the Euphrates and the Orontes, where the comparison showed lower values in the Al-Kabir Al-Shimali river environment.(author)

Medical Isotopes Production Project: Molybdenum-99 and related isotopes: Environmental Impact Statement, Volume I

International Nuclear Information System (INIS)

1996-04-01

This Environmental Impact Statement (EIS) provides environmental and technical information concerning the U.S. Department of Energy's (DOE) proposal to establish a domestic source to produce molybdenum-99 (Mo-99) and related medical isotopes (iodine-131, xenon-133 and iodine-125). Mo-99, a radioactive isotope of the element molybdenum, decays to form metastable technetium-99 (Tc-99m), a radioactive isotope used thousands of times daily in medical diagnostic procedures in the U.S. Currently, all Mo-99 used in the U.S. is obtained from a single Canadian source. DOE is pursuing the Medical Isotopes Production Project in order to ensure that a reliable supply of Mo-99 is available to the U.S. medical community. Under DOE's preferred alternative, the Chemistry and Metallurgy Research Facility at the Los Alamos National Laboratory (LANL) and the Annular Core Research Reactor and Hot Cell Facility at Sandia National Laboratories/New Mexico (SNL/NM) would be used for production of the medical isotopes. In addition to the preferred alternative, three other reasonable alternatives and a no action alternative are analyzed in detail. The sites for the three reasonable alternatives are LANL, Oak Ridge National Laboratory (ORNL), and Idaho National Engineering Laboratory (INEL). The analyses in this EIS indicate no significant difference in the potential environmental impacts among the alternatives. Each of the alternatives would use essentially the same technology for the production of the medical isotopes. Minor differences in environmental impacts among alternatives relate to the extent of activity necessary to modify and restart (as necessary) existing reactors and hot cell facilities at each of the sites, the quantities, of low-level radioactive waste generated, how such waste would be managed, and the length of time needed for initial and full production capacity

Nuclear data for unstable isotopes

International Nuclear Information System (INIS)

Sorlin, O.

1992-01-01

Nuclear Physics and Astrophysics are both entrusted with the task of understanding nucleosynthesis and energy production in the stars. At high temperatures and densities present in explosive scenarii such as the early universe, cataclysmic binary stars (nova or accretion stars), and supernovae, the nucleosynthesis proceeds throughout unstable nuclei. In order to produce and to study the most exotic isotopes that are not accessible from stable beam - stable (or radioactive) target experiments, it is necessary to develop facilities that utilize Radioactive Nuclear Beams (RNB). The existing methods for producing unstable nuclei will be described in paragraph 2. A review of the major explosive stellar processes will be made through some selected examples using RNB

Submicro and Nano Structured Porous Materials for the Production of High-Intensity Exotic Radioactive Ion Beams

CERN Document Server

Fernandes, Sandrina; Stora, Thierry

2010-01-01

ISOLDE, the CERN Isotope Separator On-line DEvice is a unique source of low energy beams of radioactive isotopes - atomic nuclei that have too many or too few neutrons to be stable. The facility is like a small ‘chemical factory’, giving the possibility of changing one element to another, by selecting the atomic mass of the required isotope beam in the mass separator, rather as the ‘alchemists’ once imagined. It produces a total of more than 1000 different isotopes from helium to radium, with half-lives down to milliseconds, by impinging a 1.4 GeV proton beam from the Proton Synchrotron Booster (PSB) onto special targets, yielding a wide variety of atomic fragments. Different components then extract the nuclei and separate them according to mass. The post-accelerator REX (Radioactive beam EXperiment) at ISOLDE accelerates the radioactive beams up to 3 MeV/u for many experiments. A wide international user radioactive ion beam (RIB) community investigates fundamental aspects of nuclear physics, particle...

Radioactive waste management: Spanish experiences

International Nuclear Information System (INIS)

Beceiro, A. R.

1996-01-01

Radioactive waste generation began in Spain during the 1950's, in association with the first applications of radioactive isotopes in industry, medicine and research. Spain's first nuclear power plant began its operations in 1968. At present, there are in operation some one thousand installations possessing the administrative authorization required to use radioactive isotopes (small producers), nine nuclear groups and a tenth is now entering the dismantling phase. There are also activities and installations pertaining to the front end of the nuclear fuel cycle (mining, milling and the manufacturing of fuel elements). Until 1985, the research center Junta de Energia Nuclear (now CIEMAT) rendered radioactive waste removal, and subsequent conditioning and temporary storage services to the small producers. Since the beginning of their operations the nuclear power plants and fuel cycle facilities have had the capacity to condition and temporarily store their own radioactive wastes. ENRESA (Empresa Nacional de Residuos Radiactivos, S. A.) began its operations in the second half of 1985. It is a state-owned company created by the Government in accordance with a previous parliamentary resolution and commissioned to establish a system for management of such wastes throughout Spain, being in charge also of the dismantling of nuclear power plants and other major installations at the end of their operating lifetimes. Possibly the most outstanding characteristic of ENRESA's evolution over these last seven years has been the need to bring about a compromise between solving the most immediate and pressing day-to-day problems of operation (the first wastes were removed at the beginning of 1986) and establishing the basic organization, resources, technology and installations required for ENRESA to operate efficiently in the long term. (author)

Radioactivity in the Marine Environment. Chapter 1

International Nuclear Information System (INIS)

Zal U'yun Wan Mahmood; Abdul Kadir Ishak; Norfaizal Mohamad; Wo, Y.M.; Kamarudin Samuding

2015-01-01

Radionuclide (radioactive isotopes or radioisotopes is widely distributed on the ground primarily in marine environments. Nowadays, more than 340 isotopes has been identified exist in our earth especially in marine environment. From that total, 80 isotopes was radioactive. The existence of radioactivity in the marine environment is through the direct and indirect distribution of radionuclides

A rich revenue from the use of radioactive beams and radioactive targets: recent highlights from the nTOF and ISOLDE facilities (1/2)

CERN Multimedia

CERN. Geneva

2008-01-01

The On-Line Isotope Mass Separator ISOLDE is a facility dedicated to the production of a large variety of radioactive ion beams for a great number of different experiments, e.g. in the field of nuclear and atomic physics, solid-state physics, life sciences and material science. At ISOLDE, radioactive nuclides are produced in thick high-temperature targets via spallation, fission or fragmentation reactions. The targets are placed in the external proton beam of the PSB, which has an energy of 1.0 or 1.4 GeV and an intensity of about 2 microA. The target and ion-source together represent a small chemical factory for converting the nuclear reaction products into a radioactive ion beam. An electric field accelerates the ions, which are mass separated and steered to the experiments. Until now more than 600 isotopes of more than 60 elements (Z=2 to 88) have been produced with half-lives down to milliseconds and intensities up to 1011 ions per second. Through the advent of post-accelerated beams with the REX-ISOLDE c...

The MOON-1 detector construction and the study of backgrounds from radioactive isotopes

International Nuclear Information System (INIS)

Ogama, T; Nakamura, H; Ejiri, H; Fushimi, K; Ichihara, K; Matsuoka, K; Nomachi, M; Hazama, R; Umehara, S; Yoshida, S; Sakiuchi, T; Hai, V H; Sugaya, Y

2006-01-01

MOON is a multilayer system of plastic scintillators and 100 Mo films for 100 Mo 0νββ decays. A prototype detector MOON-1 was built with 6 layers of plastic scintillators and 142g of 100Mo films for background (BG), energy and position resolution studies of the MOON detector. No serious BG from natural radioactive isotopes (RI) for 0νββ detection was found

Possibilities of production of neutron-rich Md isotopes in multi-nucleon transfer reactions

Energy Technology Data Exchange (ETDEWEB)

Mun, Myeong-Hwan; Lee, Young-Ouk [Korea Atomic Energy Research Institue, Daejeon (Korea, Republic of); Adamian, G.G.; Antonenko, N.V. [Joint Institute for Nuclear Research, Dubna (Russian Federation)

2016-12-15

The possibilities of production of yet unknown neutron-rich isotopes of Md are explored in several multi-nucleon transfer reactions with actinide targets and stable and radioactive beams. The projectile-target combinations and bombarding energies are suggested to produce new neutron-rich isotopes of Md in future experiments. (orig.)

44 years of testing radioactive materials packages at ORNL

Energy Technology Data Exchange (ETDEWEB)

Shappert, L.B.; Ludwig, S.B. [Oak Ridge National Lab., Oak Ridge, TN (United States)

2004-07-01

This paper briefly reviews the package testing at the Oak Ridge National Laboratory (ORNL) since 1960 and then examines the trends in the testing activities that occurred during the same period. Radioactive material shipments have been made from ORNL since the 1940s. The first fully operating reactor built at the ORNL site was patterned after the graphite pile constructed by Enrico Fermi under Stagg Field in Chicago. After serving as a test bed for future reactors, it became useful as a producer of radioactive isotopes. The Isotopes Division was established at ORNL to furnish radioactive materials used in the medical community. Often these shipments have been transported by aircraft worldwide due to the short half-lives of many of the materials. This paper touches briefly on the lighter and smaller radioisotope packages that were being shipped from ORNL in large numbers and then deals with the testing of packages designed to handle large radioactive sources, such as spent fuel, and other fissile materials.

44 years of testing radioactive materials packages at ORNL

International Nuclear Information System (INIS)

Shappert, L.B.; Ludwig, S.B.

2004-01-01

This paper briefly reviews the package testing at the Oak Ridge National Laboratory (ORNL) since 1960 and then examines the trends in the testing activities that occurred during the same period. Radioactive material shipments have been made from ORNL since the 1940s. The first fully operating reactor built at the ORNL site was patterned after the graphite pile constructed by Enrico Fermi under Stagg Field in Chicago. After serving as a test bed for future reactors, it became useful as a producer of radioactive isotopes. The Isotopes Division was established at ORNL to furnish radioactive materials used in the medical community. Often these shipments have been transported by aircraft worldwide due to the short half-lives of many of the materials. This paper touches briefly on the lighter and smaller radioisotope packages that were being shipped from ORNL in large numbers and then deals with the testing of packages designed to handle large radioactive sources, such as spent fuel, and other fissile materials

Nuclear radioactive techniques applied to materials research

CERN Document Server

Correia, João Guilherme; Wahl, Ulrich

2011-01-01

In this paper we review materials characterization techniques using radioactive isotopes at the ISOLDE/CERN facility. At ISOLDE intense beams of chemically clean radioactive isotopes are provided by selective ion-sources and high-resolution isotope separators, which are coupled on-line with particle accelerators. There, new experiments are performed by an increasing number of materials researchers, which use nuclear spectroscopic techniques such as Mössbauer, Perturbed Angular Correlations (PAC), beta-NMR and Emission Channeling with short-lived isotopes not available elsewhere. Additionally, diffusion studies and traditionally non-radioactive techniques as Deep Level Transient Spectroscopy, Hall effect and Photoluminescence measurements are performed on radioactive doped samples, providing in this way the element signature upon correlation of the time dependence of the signal with the isotope transmutation half-life. Current developments, applications and perspectives of using radioactive ion beams and tech...

Peculiarity of radioactivity pollution of manufacturing environment gas and oil producing firms of the apsheron region

International Nuclear Information System (INIS)

Mamedov, A.M.; Alekperova, J.A.

2002-01-01

Full text: Present time protection of the biosphere from technogene pollution is the important problem, having common to all mankind value. In circuits of the technogene pollution of the environment the soil is a carrying on link for through soil the contaminants freely go to air environment, in underground waters in plants and in foodstuff of a vegetative and animal genesis. In subsequent these contaminants on the indicated chains by penetrating in an organism of the people render an ill effect on their health. In this plane the radiological contamination of soil introduces still large dangerous. As the radionuclides of soil can render as external radiation, and by getting in an organism with air, water and foodstuff can cause internal radiation. In this plane, for detection of a role of gas and oil producing firms in radiological contamination soil as object of an environment, we conduct researches by a hygienic estimation of radiological contamination of soil of territory of oil-fields OOGE 'Gum adasi' of the Apsheron region. By spectrometric method were studied a natural background radiation and radioactivity of soil of different territories of shop of complex opening-up of oil. Established, that for the raw tank the specific activity reaches 4438-9967 Bk/kg, close of the product repair shop the radioactivity reached 650- 700 micro R/hour. In territory of the region 'Gum adasi', where the waste from cleaning chisel tubes were accumulated, the radioactivity made 600 micro R/hour. These indexes the superior background level is significant. The analysis of power spectrums a gamma of radiations is model from the indicated sites has shown, that the radioactivity is conditioned by isotopes of a radium. The researches have allowed to demonstrate a radioactivity technogene of impurity of rocks to recommend urgent dumping of above-stated waste in bunkers on sites, retracted by it. Thus, was established, that gas and oil producing firms contributing to radiological

Significance of iodine radioactive isotopes in the problem of radiation safety of nuclear fuel cycle

International Nuclear Information System (INIS)

Malenchenko, A.F.; Mironov, V.P.

1979-01-01

The data on actual wastes of nuclear-power plants, environmental distribution and biological effects of iodine radioactive isotopes have been analyzed. Dose-response relationship is estimated as well as its significance for struma maligna development under ionizing radiation and the contribution of iodine radionuclides resulted from nuclear power engineering to this process

Determination of radioactive scales in oil industry using naturally occurring radioactive materials

International Nuclear Information System (INIS)

Al-Masri, M. S.

2006-06-01

In the present study, naturally occurring radioactive materials (Radium isotopes) present in produced water and radiation measurements have been used to study the formation of scales, evaluate their age, determination of geological formations and between wells interactions. Produced water samples were collected and analyzed monthly for 5 months from 11 oil wells in three Syrian oil fields. Analysis includes radium isotopes and anions and cations concentrations in addition to radiation measurements at the well heads. The highest mean values of radium 226, Radium 228 and Radium 224 concentration in produced were 41 Bq/1, 57.1 Bq/1 and 1.1 Bq/1, respectively. The values obtained for Radium 226, Radium 228 and the activity ratio were statistically evaluated and the results were presented using the box plot method. The mean value of the activity ration of Radium 226 and Radium 228 was used to determine the age of scales accumulated inside tubulars. (author)

Medical Isotopes Production Project: Molybdenum-99 and related isotopes - environmental impact statement. Volume II, comment response document

International Nuclear Information System (INIS)

1996-04-01

This Environmental Impact Statement (EIS) provides environmental and technical information concerning the U.S. Department of Energy's (DOE) proposal to establish a domestic source to produce molybdenum-99 (Mo-99) and related isotopes (iodine-131, xenon-133, and iodine-125). Mo-99, a radioactive isotope of the element molybdenum, decays to form metastable technetium-99 (Tc-99m), a radioactive isotope used thousands of times daily in medical diagnostic procedures in the U.S. Currently, all Mo-99 used in the U.S. is obtained from a single Canadian source. DOE is pursuing the Medical Isotopes Production Project in order to ensure that a reliable supply of Mo-99 is available to the U.S. medical community as soon as practicable. Under DOE's preferred alternative, the Chemistry and Metallurgy Research Facility at the Los Alamos National Laboratory (LANL) and the Annular Core Research Reactor and Hot Cell Facility at Sandia National Laboratories/New Mexico (SNL/NM) would be used for production of the medical isotopes. In addition, three other reasonable alternatives and a No Action alternative are analyzed in detail, The sites for these three reasonable alternatives are LANL, Oak Ridge National Laboratory (ORNL), and Idaho National Engineering Laboratory (INEL). The analyses in this EIS indicate no significant difference in the potential environmental impacts among the alternatives. Each of the alternatives would use essentially the same technology for the production of the medical isotopes. Minor differences in environmental impacts among alternatives relate to the extent of activity necessary to modify and restart (as necessary) existing reactors and hot cell facilities at each of the sites, the quantities of low-level radioactive waste generated, how such waste would be managed, and the length of time needed for initial and full production capacity. This document contains comments recieved from meetings held regarding the site selection for isotope production

Survey of literature on the use of radioactive isotopes in agriculture published between 1973 and 1980

International Nuclear Information System (INIS)

Van der Westhuizen, M.; Van der Bank, D.J.; Van der Berg, G.W.J.; Uys, A.

1980-04-01

The literature on the use of radioactive isotopes in agriculture appears in reports and magazines which are spread over a wide spectrum of disciplines, e.g. nuclear science and agriculture science. For this reason it will be of assistance to practicing scientists to have in one volume a compilation of literature covering this field. The first part of this report consists of a list of books on this subject published by the International Atomic Energy Agency in Vienna. Most of the books are proceedings of symposia and seminars but the report also includes manuals on specialised subjects, useful for scientists starting in this field. The second part of this report consists of titles of reports and magazine articles. These were obtained form 'INIS Atomindex' for the years 1973-1980. It is hoped that the items presented in this report will be useful to scientists interested in the application of radioactive isotopes to agricultural research

Alloy development for fast induced radioactivity decay for fusion reactor applications

International Nuclear Information System (INIS)

Klueh, R.L.; Bloom, E.E.

1984-03-01

The Cr-Mo ferritic (martensitic) steels and austenitic stainless steels (primarily type 316 and variations on that composition) are the leading candidates for the structural components for future fusion reactors. However, irradiation of such steels in a fusion environment produces long-lived radioactive isotopes. These isotopes lead to difficult radioactive waste disposal problems once the structure is removed from service. Such problems could be reduced by developing steels that contain only elements that produce radioactive isotopes that decay to low levels in a reasonable time (tens of years instead of hundreds or thousands of years). This report discusses the development of such steels by making elemental substitutions in the steels now under consideration. Molybdenum must be replaced in the Cr-Mo steels; nickel and molybdenum both must be replaced in the austenitic stainless steels (the nitrogen concentration must be limited, and niobium, maintained to extremely low levels). Appropriate substitutions are tungsten for molybdenum in the Cr-Mo steels and manganese for nickel in the austenitic stainless steels. Indications are that suitable ferritic steels can be developed, but development of a nickel-free austenitic stainless steel with properties similar to the Cr-Ni stainless steels appears to be much more complex

Geochemical and strontium isotope characterization of produced waters from Marcellus Shale natural gas extraction.

Science.gov (United States)

Chapman, Elizabeth C; Capo, Rosemary C; Stewart, Brian W; Kirby, Carl S; Hammack, Richard W; Schroeder, Karl T; Edenborn, Harry M

2012-03-20

Extraction of natural gas by hydraulic fracturing of the Middle Devonian Marcellus Shale, a major gas-bearing unit in the Appalachian Basin, results in significant quantities of produced water containing high total dissolved solids (TDS). We carried out a strontium (Sr) isotope investigation to determine the utility of Sr isotopes in identifying and quantifying the interaction of Marcellus Formation produced waters with other waters in the Appalachian Basin in the event of an accidental release, and to provide information about the source of the dissolved solids. Strontium isotopic ratios of Marcellus produced waters collected over a geographic range of ~375 km from southwestern to northeastern Pennsylvania define a relatively narrow set of values (ε(Sr)(SW) = +13.8 to +41.6, where ε(Sr) (SW) is the deviation of the (87)Sr/(86)Sr ratio from that of seawater in parts per 10(4)); this isotopic range falls above that of Middle Devonian seawater, and is distinct from most western Pennsylvania acid mine drainage and Upper Devonian Venango Group oil and gas brines. The uniformity of the isotope ratios suggests a basin-wide source of dissolved solids with a component that is more radiogenic than seawater. Mixing models indicate that Sr isotope ratios can be used to sensitively differentiate between Marcellus Formation produced water and other potential sources of TDS into ground or surface waters.

Memory Effects Study of Measuring Radioactive Xenon Isotopes With β-γ Coincidence Method

International Nuclear Information System (INIS)

Jia Huaimao; Wang Shilian; Wang Jun; Li Qi; Zhao Yungang; Fan Yuanqing; Zhang Xinjun

2010-01-01

The β-γ coincidence technique is a kind of the key important method to detect radioactive xenon isotopes for the Comprehensive Nuclear-Test-Ban Treaty (CTBT). This paper describes noble gases memory effects of β-γ coincidence detector. Xenon memory effects were measured and its influence on detector's minimum detectable activity (MDA) was evaluated. The methods of reducing xenon memory effects were studied. In conclusion, aluminium coated plastic scintillator and YAP scintillator can remarkably decrease xenon memory effects. (authors)

Isotope techniques in hydrology and sedimentology

International Nuclear Information System (INIS)

Bomtempo, Virgilio Lopardi

1999-01-01

Water is the foundation of all life on Earth. Although two thirds of the terrestrial surface are covered by water (estimated volume is 1.5 billion cubic meters), just 2% of this total are fresh water, most of it locked in glaciers, ice caps and in deep groundwater reservoirs. Only 2,000 cubic kilometers are estimated to be available for consumption. Water resources have become more and more scarce, and the utilization becomes increasingly costly, due to the impact caused by over-exploitation and by diversified fronts of pollution. Specialists have been working in the development and in the application of several techniques to face this problem and to produce sustainable solutions. Isotope techniques represent a group of widespread tools that have been used along many years, and have become outstanding in hydrological investigation. This paper introduces a comprehensive review of the isotope techniques, taking into account environmental isotopes (stable and radioactive), artificial tracers and the use of radioactive sealed sources. Potentialities and limitations, future perspectives, as well as risks and benefits are also discussed. (author)

K isomerism and collectivity in neutron-rich rare-earth isotopes.

OpenAIRE

Patel, Zena

2016-01-01

Neutron-rich rare-earth isotopes were produced by in-flight fission of 238U ions at the Radioactive Isotope Beam Factory (RIBF), RIKEN, Japan. In-flight fission of a heavy, high-intensity beam of 238U ions on a light target provides the cleanest secondary beams of neutron-rich nuclei in the rare-earth region of isotopes. In-flight fission is advantageous over other methods of nuclear production, as it allows for a secondary beam to be extracted, from which the beam species can be separated an...

The reactor and the production of isotopes

International Nuclear Information System (INIS)

Hevesy, G. de

1962-01-01

The construction of the cyclotron immensely advanced the availability of radioactive tracers, a few of which even today can be produced only with the aid of this device. But even this great advance was overshadowed by the fabulous production of isotopes by the reactors. Isotopes of almost any element and of almost unlimited activity became available. It now became possible to apply H 3 - discovered already in the 'thirties by Rutherford and Oliphant - and C 14 , and these were used in thousands of investigations

High resolution laser spectroscopy of radioactive isotopes using a RFQ cooler-buncher at CERN-ISOLDE

CERN Document Server

Mané, E

2009-01-01

At CERN, the European Organization for Nuclear Research, radioactive nuclear beams are produced at the On-Line Isotope Mass Separator facility, ISOLDE. This facility provides a variety of exotic nuclear species for multidisciplinary experiments including nuclear physics. A gas-filled linear Paul trap was commissioned off-line and on-line and now is fully integrated at the focal plane of the high resolution separator magnets of ISOLDE. Ion beams with reduced transverse emitance and energy spread are now available for all experiments located downstream the separator beam line. This device is also able to accumulate the ion beam and release the collected sample in short bunches. Typical accumulation times are 100 ms and the released bunch width is 5-20 $\\mu{s}$. Such bunching capabilities has substantially increased the sensitivity of collinear laser spectroscopy with fluorescence detection by reducing the background from laser scatter by up to four orders of magnitude. The spectroscopic quadrupole moments of $^...

Nuclear structure from radioactive decay

International Nuclear Information System (INIS)

Wood, J.L.

1991-01-01

This report discusses nuclear structure from radioactive decay of the following: Neutron-Deficient Iridium Isotopes; Neutron-Deficient Platinum Isotopes; Neutron-Deficient Gold Isotopes; Neutron-Deficient Mercury Isotopes; Neutron-Deficient Thallium Isotopes; Neutron-Deficient Lead Isotopes; Neutron-Deficient Samarium Isotopes; Neutron-Deficient Promethium Isotopes; Neutron-Deficient Neodymium Isotopes; and Neutron-Deficient Praseodymium Isotopes. Also discussed are Nuclear Systematics and Models

Recycling radioactive scrap metal by producing concrete shielding with steel granules

International Nuclear Information System (INIS)

Sappok, M.

1996-01-01

Siempelkamp foundry at Krefeld, Germany, developed a method for recycling radioactively contaminated steel from nuclear installations. The material is melted and used for producing shielding plates, containers, etc., on a cast-iron basis. Because the percentage of stainless steel has recently increased significantly, problems in the production of high-quality cast iron components have also grown. The metallurgy, the contents of nickel and chromium especially, does not allow for the recycling of stainless steel in a percentage to make this process economical. In Germany, the state of the art is to use shielded concrete containers for the transport of low active waste; this concrete is produced by using hematite as an additive for increasing shielding efficiency. The plan was to produce steel granules from radioactive scrap metal as a substitute for hematite in shielding concrete

α decay and cluster radioactivity of nuclei of interest to the synthesis of Z =119 , 120 isotopes

Science.gov (United States)

Poenaru, D. N.; Gherghescu, R. A.

2018-04-01

Super-heavy nuclei of interest for the forthcoming synthesis of the isotopes with Z =119 , 120 are investigated. One of the very interesting latest experiments was performed at the velocity filter SHIP (GSI Darmstadt) trying to produce 299120 in a fusion reaction 248Cm(54Cr,3 n )299120 . We report calculations of α -decay half-lives using four models: AKRA (Akrawy), ASAF (analytical superasymmetric fission), UNIV (universal formula), and semFIS (semi-empirical formula based on fission theory). The released energy, Q , is calculated using the theoretical model of atomic masses, WS4. For Sr,9492 cluster radioactivity of 120,302300 we predict a branching ratio relative to α decay of -0.10 and 0.49, respectively, meaning that it is worth trying to detect such kinds of decay modes in competition with α decay.

Management of radioactive medical waste

International Nuclear Information System (INIS)

Deschamps, S.; Mathey, J.C.

1996-01-01

Hospitals are producers of small amounts of radioactive waste. Current legislation details exactly how hospitals should manage it. Sealed sources are returned to suppliers. Disposal of unsealed sources, liquid or solid, depends upon their half-life: short-lived radioisotopes (half-life less than two months) are stocked on site while they decay; isotopes with longer half-lives (greater than two months) are handled by a specialist organization (ANDRA). (authors). 8 refs

Production of platinum radioisotopes at Brookhaven Linac Isotope Producer (BLIP

Directory of Open Access Journals (Sweden)

Smith Suzanne V.

2017-01-01

Full Text Available The accelerator production of platinum isotopes was investigated at the Brookhaven Linac Isotope Producer (BLIP. In this study high purity natural platinum foils were irradiated at 53.2, 65.7, 105.2, 151.9, 162.9 and 173.3.MeV. The irradiated foils were digested in aqua regia and then converted to their hydrochloride salt with concentrated hydrochloric acid before analyzing by gamma spectrometry periodically for at least 10 days post end of bombardment. A wide range of platinum (Pt, gold (Au and iridium (Ir isotopes were identified. Effective cross sections at BLIP for Pt-188, Pt-189, Pt-191 and Pt-195m were compared to literature and theoretical cross sections determined using Empire-3.2. The majority of the effective cross sections (<70 MeV confirm those reported in the literature. While the absolute values of the theoretical cross sections were up to a factor of 3 lower, Empire 3.2 modeled thresholds and maxima correlated well with experimental values. Preliminary evaluation into a rapid separation of Pt isotopes from high levels of Ir and Au isotopes proved to be a promising approach for large scale production. In conclusion, this study demonstrated that with the use of isotopically enriched target material accelerator production of selected platinum isotopes is feasible over a wide proton energy range.

Source term estimation and the isotopic ratio of radioactive material released from the WIPP repository in New Mexico, USA

International Nuclear Information System (INIS)

Thakur, P.

2016-01-01

After almost 15 years of operations, the Waste Isolation Pilot Plant (WIPP) had one of its waste drums breach underground as a result of a runaway chemical reaction in the waste it contained. This incident occurred on February 14, 2014. Moderate levels of radioactivity were released into the underground air. A small portion of the contaminated underground air also escaped to the surface through the ventilation system and was detected approximately 1 km away from the facility. According to the source term estimation, the actual amount of radioactivity released from the WIPP site was less than 1.5 mCi. The highest activity detected on the surface was 115.2 μBq/m 3 for 241 Am and 10.2 μBq/m 3 for 239+240 Pu at a sampling station located 91 m away from the underground air exhaust point and 81.4 μBq/m 3 of 241 Am and 5.8 μBq/m 3 of 239+240 Pu at a monitoring station located approximately 1 km northwest of the WIPP facility. The dominant radionuclides released were americium and plutonium, in a ratio that matches the content of the breached drum. Air monitoring across the WIPP site intensified following the first reports of radiation detection underground to determine the extent of impact to WIPP personnel, the public, and the environment. In this paper, the early stage monitoring data collected by an independent monitoring program conducted by the Carlsbad Environmental Monitoring & Research Center (CEMRC) and an oversight monitoring program conducted by the WIPP's management and operating contractor, the Nuclear Waste Partnership (NWP) LLC were utilized to estimate the actual amount of radioactivity released from the WIPP underground. The Am and Pu isotope ratios were measured and used to support the hypothesis that the release came from one drum identified as having breached that represents a specific waste stream with this radionuclide ratio in its inventory. This failed drum underwent a heat and gas producing reaction that overpowered its vent and

Techniques and problems in studying intestinal absorption with radioactive isotopes in children

International Nuclear Information System (INIS)

James, W.P.T.; Waterlow, J.C.

1976-01-01

Radioactive isotopes give substantial promise for assisting the study of gastrointestinal absorption in children in that they allow reduction or elimination of the collection of blood, urine and faeces specimens. These operations are particularly difficult and unreliable in infants, on whom greatest interest in paediatric gastroenterology is centred in the tropics. Here intestinal malabsorption is most commonly associated with malnutrition, lactose intolerance, gastroenteritis, parasitic infestation and iron-deficiency anaemia. Two general techniques that have been employed are whole-body counting and analyses of 14 CO 2 exhaled in the breath after the feeding of 14 C-labelled nutrients. The former is advantageous if radionuclides suitable for the test at hand exist; the latter may be hard to interpret because of problems in the distribution and metabolism of the nutrient and intermediary products. Proper selection and understanding of the tests is particularly important in paediatric work, where the use of radioactive tracer techniques is unacceptable merely for the convenience of the investigator. (author)

Ion beam production and study of radioactive isotopes with the laser ion source at ISOLDE

Science.gov (United States)

Fedosseev, Valentin; Chrysalidis, Katerina; Day Goodacre, Thomas; Marsh, Bruce; Rothe, Sebastian; Seiffert, Christoph; Wendt, Klaus

2017-08-01

At ISOLDE the majority of radioactive ion beams are produced using the resonance ionization laser ion source (RILIS). This ion source is based on resonant excitation of atomic transitions by wavelength tunable laser radiation. Since its installation at the ISOLDE facility in 1994, the RILIS laser setup has been developed into a versatile remotely operated laser system comprising state-of-the-art solid state and dye lasers capable of generating multiple high quality laser beams at any wavelength in the range of 210-950 nm. A continuous programme of atomic ionization scheme development at CERN and at other laboratories has gradually increased the number of RILIS-ionized elements. At present, isotopes of 40 different elements have been selectively laser-ionized by the ISOLDE RILIS. Studies related to the optimization of the laser-atom interaction environment have yielded new laser ion source types: the laser ion source and trap and the versatile arc discharge and laser ion source. Depending on the specific experimental requirements for beam purity or versatility to switch between different ionization mechanisms, these may offer a favourable alternative to the standard hot metal cavity configuration. In addition to its main purpose of ion beam production, the RILIS is used for laser spectroscopy of radioisotopes. In an ongoing experimental campaign the isotope shifts and hyperfine structure of long isotopic chains have been measured by the extremely sensitive in-source laser spectroscopy method. The studies performed in the lead region were focused on nuclear deformation and shape coexistence effects around the closed proton shell Z = 82. The paper describes the functional principles of the RILIS, the current status of the laser system and demonstrated capabilities for the production of different ion beams including the high-resolution studies of short-lived isotopes and other applications of RILIS lasers for ISOLDE experiments. This article belongs to the Focus on

Guide book of radioactive wastes collecting. Producers, from collection to storage

International Nuclear Information System (INIS)

2003-01-01

This document, more particularly devoted to radioactive waste producers (except electronuclear industry), defines the technical specifications and the financial conditions relative to the taking over of their wastes by the ANDRA, the French national agency of radioactive wastes. Content: general principles, instructions manual of the taking over demand, practical conditions of wastes collecting, packaging and containers, specifications for each category of waste, particular cases, price table, disputes. (J.S.)

Asymptotic giant branch stars as producers of carbon and of neutron-rich isotopes

International Nuclear Information System (INIS)

Iben, I. Jr.

1984-01-01

Carbon stars are thought to be in the asymptotic giant branch (AGB) phase of evolution, alternately burning hydrogen and helium in shells above an electron-degenerate carbon-oxygen (CO) core. The excess of carbon relative to oxygen at the surfaces of these stars is thought to be due to convective dredge-up which occurs following a thermal pulse. During a thermal pulse, carbon and neutron-rich isotopes are made in a convective helium-burning zone. In model stars of large CO core mass, the source of neutrons for producing the neutron-rich isotopes is the 22 Ne(α,n) 25 Mg reaction and the isotopes are produced in the solar system s-process distribution. In models of small core mass, the 13 C(α,n) 16 reaction is thought to be responsible for the release of neutrons, and the resultant distribution of neutron-rich isotopes is expected to vary considerably from one star to the next, with the distribution in isolated instances possibly resembling the solar system distribution of r-process isotopes

2. Workshop 'Isotopes in Nature'. 1

International Nuclear Information System (INIS)

1979-11-01

The workshop was aimed at discussing in detail the following problems: (1) distribution of stable and radioactive isotopes in nature, (2) theoretical and experimental studies of isotopic effects in natural processes, (3) problems of sample preparation and sample measurement in determining the relative abundance of stable isotopes or radioactive isotopes in nature, (4) age estimations of samples from different areas of the geosphere, (5) contributions to the specification of global and regional substance cycles in nature with the aid of isotopic and geochemical studies. 75 summaries are included

The future of producing separated stable isotopes at Oak Ridge National Laboratory for accelerator applications

International Nuclear Information System (INIS)

Collins, E.D.

1994-01-01

Separated stable isotopes, produced in the calutrons at Oak Ridge National Laboratory, are essential target materials for production of numerous radioisotopes in accelerators and reactors. Recently, separated stable isotope production has been curtailed because government appropriations were discontinued and salts revenues decreased. The calutrons were placed in standby and the operating staff reduced to enable support by sales from existing inventories. Appeals were made to industry and government to preserve this national capability. Methods for providing volume-based price reductions were created to attract support from commercial isotope users. In 1994, the Department of Energy's Isotope Production and Distribution Program was restructured and a strategy produced to seek appropriated funding for the future production of rare, nonprofitable isotopes for research uses. This strategy, together with new demands for medical isotopes, will enable future operation of the calutrons. Moreover, production may be enhanced by complementing calutron capabilities with the Plasma Separation Process

Isotope toolbox turns 10

DEFF Research Database (Denmark)

Wenander, Fredrik; Riisager, Karsten

2012-01-01

REX-ISOLDE, one of CERN’s most compact accelerators, has just celebrated its 10th anniversary. The machine’s versatility provides radioactive ion beams across the range of nuclear isotopes.......REX-ISOLDE, one of CERN’s most compact accelerators, has just celebrated its 10th anniversary. The machine’s versatility provides radioactive ion beams across the range of nuclear isotopes....

Radioactive sources production in the Boris Kidric Institute of nuclear sciences

International Nuclear Information System (INIS)

Radosavljevic, B.; Nemoda, Dj.; Memedovic, T.; Bircanin, LJ.

1978-01-01

Since 1960, in the Laboratory for radioisotopes production of the Institute isotopes were produced for industrial, medical and research purposes. From the beginning, this activity was developed in two directions: 1. sealed sources, for industrial radiography, teletherapy Cobalt, later for lightning arresters, level meters, densitometers etc., 2. radioactive sources that need chemical treatment for different applications in industry and research. This paper lists the types of radioactive sources and methods for production [sr

Canada's isotope crisis : what next?

International Nuclear Information System (INIS)

Nathwani, J.; Wallace, D.

2010-01-01

Canada urgently requires a rigorous debate on the strategic options for ensuring a robust, reliable, and affordable supply of radioactive isotopes. Should the debate be confined to how Canada can best develop the necessary technologies solely for our own use or should Canada abandon the idea of producing its own isotope supply and any future aspirations to serve the global market? Canada's Isotope Crisis focuses on the central policy question: do we dare to try to shape the future or do we retreat into silence because we are not prepared to make the necessary investments for the future well-being of Canadians? This volume showcases pointed essays and analysis from members of the academy and individuals who have made contributions to the development of medical isotopes and pioneered their use in medical practice. It also includes commentary from those involved in the production, manufacturing, processing, and distribution of isotopes. Canada's Isotope Crisis is a multi-disciplinary effort that addresses the global dimension of isotope supply and combines expert opinions on the present and past with knowledge of the relevant government agencies and the basis for their decisions at critical junctures.

Development of an externally controllable sealed isotope generator.

Science.gov (United States)

Sasaki, Toru; Aoki, Katsumi; Yamashita, Ryosuke; Hori, Kensuke; Kato, Taiga; Saito, Misaki; Niisawa, Kazuhiro; Nagatsu, Kotaro; Nozaki, Tadashi

2018-03-01

An externally controllable sealed isotope generator has been proposed for radiation education activities. Column ( 68 Ge- 68 Ga and 137 Cs- 137m Ba) and solvent extraction ( 68 Ge- 68 Ga)-based isotope generators were applied as radioactive sources. These generators showed high milking efficiencies and low breakthrough after repeated uses, and are expected to promote the use of isotope generators without radioactive contamination or the emission of radioactive waste. This isotope generator provides a new concept for sealed radioisotope sources. Copyright © 2017 Elsevier Ltd. All rights reserved.

Laser-spectroscopic nuclear-structure studies on radioactive silver and indium isotopes

International Nuclear Information System (INIS)

Dinger, U.

1988-05-01

Neutron-deficient silver and neutron-rich indium isotopes were studied by collinear laser spectroscopy. The neutron-deficient nuclei 101 , 103 , 104 , 105 , 105m , 106m Ag were produced as evaporation-residual nuclei in heavy-ion fusion reactions at the mass separator of the GSI in Darmstadt. The fourteen studied indium isotopes and isomers with even mass number in the range 112-126 In were produced by 600-MeV-proton induced fission of a uranium carbide target at the ISOLDE separator in Geneva. The mass-separated ion beam was subsequently deviated electrostatically, neutralized in a sodium vapor and superposed with a c w dye laser. A photon counting system detected the resonance fluorescence of the induced transitions. The hyperfine structure and the isotope shift of the 4d 9 5s 2 2 D 5/2 → 4d 10 6p 2 P 3/2 transition (λ=547.7 nm) in silver and the 5p 2 P 1/2,3/2 → 6s 2 s 1/2 transition (λ=410 respectively 451 nm) in indium were measured. While in indium for the analysis of the data earlier work could be referred to, in silver a detailed analysis of the isotope shift and hyperfine structure was performed by means of ab initio calculations and semi-empirical procedures. Thereby the configuration interactions were especially considered. The nuclear moments were discussed in the framework of existing nuclear models regarding nuclear-spectroscopic informations. (orig./HSI) [de

Isotopes a very short introduction

CERN Document Server

Ellam, Rob

2016-01-01

An isotope is a variant form of a chemical element, containing a different number of neutrons in its nucleus. Most elements exist as several isotopes. Many are stable while others are radioactive, and some may only exist fleetingly before decaying into other elements. In this Very Short Introduction, Rob Ellam explains how isotopes have proved enormously important across all the sciences and in archaeology. Radioactive isotopes may be familiar from their use in nuclear weapons, nuclear power, and in medicine, as well as in carbon dating. They have been central to establishing the age of the Earth and the origins of the solar system. Combining previous and new research, Ellam provides an overview of the nature of stable and radioactive isotopes, and considers their wide range of modern applications. ABOUT THE SERIES: The Very Short Introductions series from Oxford University Press contains hundreds of titles in almost every subject area. These pocket-sized books are the perfect way to get ahead in a new subjec...

Factors that control the stable carbon isotopic composition of methane produced in an anoxic marine sediment

Science.gov (United States)

Alperin, M. J.; Blair, Neal E.; Albert, D. B.; Hoehler, T. M.; Martens, C. S.

1993-01-01

The carbon isotopic composition of methane produced in anoxic marine sediment is controlled by four factors: (1) the pathway of methane formation, (2) the isotopic composition of the methanogenic precursors, (3) the isotope fractionation factors for methane production, and (4) the isotope fractionation associated with methane oxidation. The importance of each factor was evaluated by monitoring stable carbon isotope ratios in methane produced by a sediment microcosm. Methane did not accumulate during the initial 42-day period when sediment contained sulfate, indicating little methane production from 'noncompetitive' substrates. Following sulfate depletion, methane accumulation proceeded in three distinct phases. First, CO2 reduction was the dominant methanogenic pathway and the isotopic composition of the methane produced ranged from -80 to -94 per thousand. The acetate concentration increased during this phase, suggesting that acetoclastic methanogenic bacteria were unable to keep pace with acetate production. Second, acetate fermentation became the dominant methanogenic pathway as bacteria responded to elevated acetate concentrations. The methane produced during this phase was progressively enriched in C-13, reaching a maximum delta(C-13) value of -42 per thousand. Third, the acetate pool experienced a precipitous decline from greater than 5 mM to less than 20 micro-M and methane production was again dominated by CO2 reduction. The delta(C-13) of methane produced during this final phase ranged from -46 to -58 per thousand. Methane oxidation concurrent with methane production was detected throughout the period of methane accumulation, at rates equivalent to 1 to 8 percent of the gross methane production rate. Thus methane oxidation was too slow to have significantly modified the isotopic signature of methane. A comparison of microcosm and field data suggests that similar microbial interactions may control seasonal variability in the isotopic composition of methane

Spatial distribution sampling and Monte Carlo simulation of radioactive isotopes

CERN Document Server

Krainer, Alexander Michael

2015-01-01

This work focuses on the implementation of a program for random sampling of uniformly spatially distributed isotopes for Monte Carlo particle simulations and in specific FLUKA. With FLUKA it is possible to calculate the radio nuclide production in high energy fields. The decay of these nuclide, and therefore the resulting radiation field, however can only be simulated in the same geometry. This works gives the tool to simulate the decay of the produced nuclide in other geometries. With that the radiation field from an irradiated object can be simulated in arbitrary environments. The sampling of isotope mixtures was tested by simulating a 50/50 mixture of $Cs^{137}$ and $Co^{60}$. These isotopes are both well known and provide therefore a first reliable benchmark in that respect. The sampling of uniformly distributed coordinates was tested using the histogram test for various spatial distributions. The advantages and disadvantages of the program compared to standard methods are demonstrated in the real life ca...

Production of adsorbent from palm shell for radioactive iodine scrubbing process

International Nuclear Information System (INIS)

Mohamad Azman Che Mat Isa; Ku Halim Ku Hamid; Muhd Noor Muhd Yunus; Mohamad Puad Abu; Abdul Halim Badaruddin; Mohammad Nizammudin Abd Aziz; Muhd Ridwan Abdul Rahim

2010-01-01

The biggest biomass source in Malaysia comes from oil palm industry. According to the statistic of year 2004, Malaysia produced 40 million tones per year of biomass which 30 million tones of biomass originated from the oil palm industries. Therefore, the biomass waste such as palm kernel shell can be used to produce granular adsorbent for radioactive materials. For that reason, a newly system, called Rocking Kiln - Fluidized Bed (RK - FB) was developed to utilize large amount of the biomass to produce high value added product. Charcoal or chemically produced activated carbon could be produced by using the kiln. Washing process was introduced to remove particles, minerals and volatile matters from charcoal produced and then would create more surface area in the adsorbent by creating more active sites. In this research, the adsorbent produced was used to scrub iodine 131. In nuclear power reactor, iodine isotope 131 is produced during nuclear fission, and this elementary radioactive iodine may pollute exhaust air streams that could cause thyroid cancer. For removal of radioactive iodine, normally a potassium iodide - impregnated activated carbon (KI - AC) is used. Thus, a process will be developed to produce KI - AC and this product will be used to calculate the efficiency to remove the radioactive iodine 131.The results obtain show that adsorbent produced has a high potential to be used in radioactive adsorbing and likely more economics. This paper will elaborate further the experimental set-up of in Kiln - Fluidized Bed (RK - FB), adsorbent quality and radioactive scrubbing process. (author)

Cooling of radioactive isotopes for Schottky mass spectrometry

International Nuclear Information System (INIS)

Steck, M.; Beckert, K.; Eickhoff, H.; Franzke, B.; Nolden, F.; Reich, H.; Schlitt, B.; Winkler, T.

1999-01-01

Nuclear masses of radioactive isotopes can be determined by measurement of their revolution frequency relative to the revolution frequency of reference ions with well-known masses. The resolution of neighboring frequency lines and the accuracy of the mass measurement is dependent on the achievable minimum longitudinal momentum spread of the ion beam. Electron cooling allows an increase of the phase space density by several orders of magnitude. For high intensity beams Coulomb scattering in the dense ion beam limits the beam quality. For low intensity beams a regime exists in which the diffusion due to intrabeam scattering is not dominating any more. The minimum momentum spread δp/p=5x10 -7 which is observed by Schottky noise analysis is considerably higher than the value expected from the longitudinal electron temperature. The measured frequency spread results from fluctuations of the magnetic field in the storage ring magnets. Systematic mass measurements have started and can be presently used for ions with half-lives of some ten seconds. For shorter-lived nuclei a stochastic precooling system is in preparation

Centralized treatment facility for low level radioactive waste produced in Belgium. The CILVA project

International Nuclear Information System (INIS)

Renard, Cl.; Detilleux, M.; Debieve, P.

1993-01-01

Due to rather limited amount of waste produced and the small size of the Belgian territory (30 x 10 3 km 2 ), ONDRAF/NIRAS strategy aims at centralizing treatment conditioning and storage of radioactive waste. ONDRAF/NTRAS has decided to set up a new infrastructure: the CILVA unit. The CILVA facility is focused on the supercompaction and the incineration treatment, so that ONDRAF/NIRAS can safely manage all radioactive wastes produced in Belgium. (2 figs.)

The South African isotope facility project

Science.gov (United States)

Bark, R. A.; Barnard, A. H.; Conradie, J. L.; de Villiers, J. G.; van Schalkwyk, P. A.

2018-05-01

The South African Isotope Facility (SAIF) is a project in which iThemba LABS plans to build a radioactive-ion beam (RIB) facility. The project is divided into the Accelerator Centre of Exotic Isotopes (ACE Isotopes) and the Accelerator Centre for Exotic Beams (ACE Beams). For ACE Isotopes, a high-current, 70 MeV cyclotron will be acquired to take radionuclide production off the existing Separated Sector Cyclotron (SSC). A freed up SSC will then be available for an increased tempo of nuclear physics research and to serve as a driver accelerator for the ACE Beams project, in which protons will be used for the direct fission of Uranium, producing beams of fission fragments. The ACE Beams project has begun with "LeRIB" - a Low Energy RIB facility, now under construction. In a collaboration with INFN Legnaro, the target/ion-source "front-end" will be a copy of the front-end developed for the SPES project. A variety of targets may be inserted into the SPES front-end; a uranium-carbide target has been designed to produce up to 2 × 1013 fission/s using a 70 MeV proton beam of 150 µA intensity.

Simulation Studies of Diffusion-Release and Effusive-Flow of Short-Lived Radioactive Isotopes

CERN Document Server

Zhang, Yan; Kawai, Yoko

2005-01-01

Delay times associated with diffusion release from targets and effusive-flow transport of radioactive isotopes to ion sources are principal intensity limiters at ISOL-based radioactive ion beam facilities, and simulation studies with computer models are cost effective methods for designing targets and vapor transport systems with minimum delay times to avoid excessive decay losses of short lived ion species. A finite difference code, Diffuse II, was recently developed at the Oak Ridge National Laboratory to study diffusion-release of short-lived species from three principal target geometries. Simulation results are in close agreement with analytical solutions to Fick’s second equation. Complementary to the development of Diffuse II, the Monte-Carlo code, Effusion, was developed to address issues related to the design of fast vapor transport systems. Results, derived by using Effusion, are also found to closely agree with experimental measurements. In this presentation, the codes will be used in conc...

Enhancing atom densities in solid hydrogen by isotopic substitution

International Nuclear Information System (INIS)

Collins, G.W.; Souers, P.C.; Mapoles, E.R.; Magnotta, F.

1991-01-01

Atomic hydrogen inside solid H 2 increases the energy density by 200 MegaJoules/m 3 , for each percent mole fraction stored. How many atoms can be stored in solid hydrogen? To answer this, we need to know: (1) how to produce and trap hydrogen atoms in solid hydrogen, (2) how to keep the atoms from recombining into the ground molecular state, and (3) how to measure the atom density in solid hydrogen. Each of these topics will be addressed in this paper. Hydrogen atoms can be trapped in solid hydrogen by co-condensing atoms and molecules, external irradiation of solid H 2 , or introducing a radioactive impurity inside the hydrogen lattice. Tritium, a heavy isotope of hydrogen, is easily condensed as a radioactive isotopic impurity in solid H 2 . Although tritium will probably not be used in future rockets, it provides a way of applying a large, homogenious dose to solid hydrogen. In all of the data presented here, the atoms are produced by the decay of tritium and thus knowing how many atoms are produced from the tritium decay in the solid phase is important. 6 refs., 6 figs

Method of producing a solution of radioactive lanthanum-140 from radioactive barium-140 in an isotope generator and installation to carry out the method

International Nuclear Information System (INIS)

Akerman, K.; Jacobs, G.; Sauerwein, K.

1979-01-01

A method of separating radioactive lanthanum-140 from radioactive Ba-140 is proposed. The lanthanum-140 will be washed out of a sulphate precipitate and separated from Ba-140-sulphate by a granular filter mass of CaSO 4 and BaSO 4 . Details of the process are given. (UWI) [de

A new approach to characterize very-low-level radioactive waste produced at hadron accelerators

International Nuclear Information System (INIS)

Zaffora, Biagio; Magistris, Matteo; Chevalier, Jean-Pierre; Luccioni, Catherine; Saporta, Gilbert; Ulrici, Luisa

2017-01-01

Radioactive waste is produced as a consequence of preventive and corrective maintenance during the operation of high-energy particle accelerators or associated dismantling campaigns. Their radiological characterization must be performed to ensure an appropriate disposal in the disposal facilities. The radiological characterization of waste includes the establishment of the list of produced radionuclides, called “radionuclide inventory”, and the estimation of their activity. The present paper describes the process adopted at CERN to characterize very-low-level radioactive waste with a focus on activated metals. The characterization method consists of measuring and estimating the activity of produced radionuclides either by experimental methods or statistical and numerical approaches. We adapted the so-called Scaling Factor (SF) and Correlation Factor (CF) techniques to the needs of hadron accelerators, and applied them to very-low-level metallic waste produced at CERN. For each type of metal we calculated the radionuclide inventory and identified the radionuclides that most contribute to hazard factors. The methodology proposed is of general validity, can be extended to other activated materials and can be used for the characterization of waste produced in particle accelerators and research centres, where the activation mechanisms are comparable to the ones occurring at CERN. - Highlights: • We developed a radiological characterization process for radioactive waste produced at particle accelerators. • We used extensive numerical experimentations and statistical analysis to predict a complete list of radionuclides in activated metals. • We used the new approach to characterize and dispose of more than 420 t of very-low-level radioactive waste.

Production of exotic, short lived carbon isotopes in ISOL-type facilities

CERN Document Server

Franberg, Hanna; Köster, Ulli; Ammann, Markus

2008-01-01

The beam intensities of short-lived carbon isotopes at Isotope Separation On-Line (ISOL) facilities have been limited in the past for technical reasons. The production of radioactive ion beams of carbon isotopes is currently of high interest for fundamental nuclear physics research. To produce radioactive ions a target station consisting of a target in a container connected to an ion source via a transfer line is commonly used. The target is heated to vaporize the product for transport. Carbon in elementary form is a very reactive element and react strongly with hot metal surfaces. Due to the strong chemisorption interaction, in the target and ion source unit, the atoms undergo significant retention on their way from the target to the ion source. Due to this the short lived isotopes decays and are lost leading to low ion yields. A first approach to tackle these limitations consists of incorporating the carbon atoms into less reactive molecules and to use materials for the target housing and the transfer line ...

World new facilities for radioactive isotope beams

International Nuclear Information System (INIS)

Motobayashi, T.

2014-01-01

The use of unstable nuclei in the form of energetic beams for nuclear physics studies is now entering into a new era. 'New-generation' facilities are either in operation, under construction or being planned. They are designed to provide radioactive isotope (RI) beams with very high intensities over a wide range of nuclides. These facilities are expected to provide opportunities to study nuclear structure, astrophysical nuclear processes and nuclear matter with large proton-neutron imbalance in grate detail. This article reports on the current status of such new-generation RI-beam facilities around the world. In order to cover different energy domains and to meet various scientific demands, the designs of RI-beam facilities are of a wide variety. For example, RIBF in Japan, FAIR in Germany and FRIB in US are based on the fragmentation scheme for beams with energies of a few hundred MeV/nucleon to GeV/nucleon, whereas Spiral2 in France, SPES in Italy, HIE-ISOLDE in Switzerland/France, and the future facility EURISOL in Europe are based on the ISOL method, and aim at providing lower-energy RI beams. There are a many other projects including upgrades of existing facilities in the three continents, America, Asia and Europe

Method of producing radioactive technetium-99M

International Nuclear Information System (INIS)

Karageozian, H.L.

1979-01-01

A chromatographic process of producing high purity and high yield radioactive Technetium-99m. A solution containing Molybdenum-99m and Technetium-99m is placed on a chromatographic column and eluted with a neutral solvent system comprising an organic solvent and from about 0.1 to less than about 10% of water or from about 1 to less than about 70% of a solvent selected from the group consisting of aliphatic alcohols having 1 to 6 carbon atoms. The eluted solvent system containing the Technetium-99m is then removed leaving the Technetium-99m as a dry, particulate residue

Development and application of RP-HPLC methods for the analysis of transition metals and their radioactive isotops in radioactive waste

International Nuclear Information System (INIS)

Seekamp, S.

1999-07-01

A major criterion in the final disposal of nuclear waste is to keep possible changes in the geosphere due to the introduction of radioactive waste as small as possible and to prevent any escape into the biosphere in the long term. The Federal Office for Radiation Protection (BfS) has therefore established limit values for a number of nuclides. Verifying these limits has to date involved laborious wet chemical analysis. In order to accelerate quantification there is a need to develop rapid multielement methods. HPLC methods represent a starting point for this development. Chemical separation is necessary to quantify β-emitters via their radioactive radiation since they are characterized by a continuous energy spectrum. A method for quantifying transition metals and their radioactive isotopes from radioactive waste has been created by using a chelating agent to select the analytes and RP-HPLC to separate the complexes formed. In addition to separating the matrix, complexation on a precolumn has the advantage of enriching the analytes. The subject of this thesis is the development and application of the method including studies of the mobile and stationary phase, as well as the optimization of all parameters, such as pH value, sample volume etc., which influence separation, enrichment or detection. The method developed was successfully tested using cement samples. It was also used for investigations of ion exchange resins and for trace analysis in calcium fluoride. Furthermore, the transferability of the method to actinides was examined by using a different complexing agent. (orig.) [de

Fuzzy rule-based modelling for human health risk from naturally occurring radioactive materials in produced water

International Nuclear Information System (INIS)

Shakhawat, Chowdhury; Tahir, Husain; Neil, Bose

2006-01-01

Produced water, discharged from offshore oil and gas operations, contains chemicals from formation water, condensed water, and any chemical added down hole or during the oil/water separation process. Although, most of the contaminants fall below the detection limits within a short distance from the discharge port, a few of the remaining contaminants including naturally occurring radioactive materials (NORM) are of concern due to their bioavailability in the media and bioaccumulation characteristics in finfish and shellfish species used for human consumption. In the past, several initiatives have been taken to model human health risk from NORM in produced water. The parameters of the available risk assessment models are imprecise and sparse in nature. In this study, a fuzzy possibilistic evaluation using fuzzy rule based modeling has been presented. Being conservative in nature, the possibilistic approach considers possible input parameter values; thus provides better environmental prediction than the Monte Carlo (MC) calculation. The uncertainties of the input parameters were captured with fuzzy triangular membership functions (TFNs). Fuzzy if-then rules were applied for input concentrations of two isotopes of radium, namely 226 Ra, and 228 Ra, available in produced water and bulk dilution to evaluate the radium concentration in fish tissue used for human consumption. The bulk dilution was predicted using four input parameters: produced water discharge rate, ambient seawater velocity, depth of discharge port and density gradient. The evaluated cancer risk shows compliance with the regulatory guidelines; thus minimum risk to human health is expected from NORM components in produced water

Iodine isotopes and radiation safety

International Nuclear Information System (INIS)

Styro, B.; Nedvekajte, T.; Filistovich, V.

1992-01-01

Methods of concentration determination of stable and radioactive iodine isotopes in the Earth's different geospheres are described. Iodine isotopes concentration data, chemical forms and transformations as well as their exchange among separate geospheres of their global biochemical circulation (ocean, atmosphere, lithosphere and biosphere) are presented. Information on iodine isotopes as after-effects of nuclear installations accident (in particular, the Chernobyl accident) is generalized. The book is intended for scientists and practical workers in ecology and radioactivity protection and for a students of physics. 442 refs.; 82 figs.; 36 tabs

Direct isotope ratio measurement of uranium metal by emission spectrometry on a laser-produced plasma

International Nuclear Information System (INIS)

Pietsch, W.; Petit, A.; Briand, A.

1995-01-01

The method of Optical Emission Spectrometry on a Laser-Produced Plasma (OES/LPP) at reduced pressure has been studied for the determination of the uranium isotope ratio ( 235 U/ 238 U). Spectral profiles of the investigated transition U-II 424.437 nm show the possibility to obtain an isotopic spectral resolution in a laser-produced plasma under exactly defined experimental conditions. Spectroscopic data and results are presented. (author)

Some applications of natural radioactivity in industry and agriculture

International Nuclear Information System (INIS)

Ma Yonghe; Xu Qiujing

1992-01-01

There are natural radioactivity isotopes of uranium, thorium and potassium everywhere in nature. The characteristics of these isotopes form the basis of various applications. Some applications of natural radioactivity in industry and agriculture are introduced

Wrong low level radioactive waste management in hospitals and improvement steps

International Nuclear Information System (INIS)

Keren, M.

2000-01-01

Hospitals are producers of great amounts of all kind of waste, including dangerous waste. The dangerous waste can be toxic, biological, radioactive, or a mixture of several kinds. There are clear procedures how to store and treat every kind of waste separately, according to its characteristics. Radioactive waste should be disposed only to a central radwaste disposal site. If the radioactive waste is mixed with biological waste, and contains long half-life isotopes, it should be neutralized from biological hazards before disposal to radwaste storage site. If the waste contains short half-life isotopes, it should be stored in a proper intermediate storage facility till a complete decay of the radioactive elements, and then treated as not radioactive. The existing procedures are old and a new proposal for radwaste procedures was prepared but not implemented. After several repetitive violations of the old regulations by some hospitals, it was decided to advance the implementation of the new proposal. This proposal consists of a detailed procedures for segregation, storage, decay and disposal of radwaste. It is based on the new recommendations of the IAEA. The responsibility for implementing the regulations is on the producers of the waste. This paper summarizes the violations and describes the main recommendations for improving procedures. The competent authority used moderate enforcement steps because of the delay in the implementation of the new procedures. As a matter of fact, the competent authority concluded that it's own investigation procedures should improve, but we shall not discuss it in this paper. (author)

Marine Biogenic Minerals Hold Clues About Changes in Ocean Chemistry and Climate: Some Important Lessons Learned from Studies of Stable and Radioactive Isotopes of Be and Al

Directory of Open Access Journals (Sweden)

Devendra Lal

2002-01-01

Full Text Available The elements Be and Al exhibit very short residence time in ocean waters, and therefore serve as useful tracers for the study of biogeochemical processes in seawater. A unique feature of these tracers is that nuclear interactions of cosmic rays in the atmosphere produce appreciable amounts of two radioactive isotopes, 10Be (with a half-life of 1.5 my and 26Al (with a half-life of 0.7 my, which are introduced in the hydrosphere, cryosphere, and lithosphere via precipitation. Thus, these elements are labeled by their respective radioactive isotopes, which help quantitative tagging of their biogeochemical cycles. Finally, as we report here, several marine organisms incorporate them in their skeletal shells in certain fixed proportions to their concentrations in the seawater, so that it seems possible to study changes in the ocean chemistry and climate over the past several million years. We summarize here the recent discovery by Dong et al.[9] of significant enrichments of intrinsic Be and Al in marine foraminiferal calcite and coral aragonite, and of Al in opal (radiolarians and aragonite (corals, which should make it possible to determine 10Be/Be and 26Al/Al in oceans in the past. We also summarize their measured 10Be/9Be in foraminiferal calcite in Pacific Ocean cores, which reveal that the concentrations and ratios of the stable and cosmogenic isotopes of Be and Al have varied significantly in the past 30 ky. The implications of these results are discussed.

Isotope hydrology: A historical overview of achievements

International Nuclear Information System (INIS)

1997-01-01

The IAEA's efforts in the water sector cover all aspects of the three main categories of isotope methodologies, such as the use of radioactive isotopes as tracers for site-specific investigations related to water movement; the use of sealed radioactive sources for in-situ measurement of hydrological field parameters; and the use of naturally occurring isotopic species for the assessment and study of water occurrence, genesis and flow pathways/dynamics at regional-scale hydrological systems

Exhaust gas cleaning system for handling radioactive fission and activation gases

International Nuclear Information System (INIS)

Queiser, H.; Schwarz, H.

1975-01-01

An exhaust gas cleaning system utilizing the principle of delaying radioactive gases to permit their radioactive decay to a level acceptable for release to the atmosphere, comprising an adsorbent for adsorbing radioactive gas and a container for containing the adsorbent and for constraining gas to flow through the adsorbent, the adsorbent and the container forming simultaneously an adsorptive delay section and a mechanical delay section, by means of a predetermined ratio of volume of voids in the adsorbent to total volume of the container containing the adsorbent, for delaying radioactive gas to permit its radioactive decay to a level acceptable for release to the atmosphere is described. A method of using an adsorbent for cleaning a radioactive gas containing an isotope which is adsorbed by the adsorbent and containing an isotope whose adsorption by the adsorbent is low as compared to the isotope which is adsorbed and which is short-lived as compared to the isotope which is adsorbed, comprising constraining the gas to flow through the adsorbent with the retention time for the isotope which is adsorbed being at least the minimum for permitting radioactive decay to a level acceptable for release to the atmosphere and with the retention time for the isotope of relatively low adsorption and relatively short life being at least the minimum for permitting radioactive decay to a level acceptable for release to the atmosphere is also described. (U.S.)

Use of radioanalytical methods for determination of uranium, neptunium, plutonium, americium and curium isotopes in radioactive wastes

International Nuclear Information System (INIS)

Geraldo, Bianca

2012-01-01

Activated charcoal is a common type of radioactive waste that contains high concentrations of fission and activation products. The management of this waste includes its characterization aiming the determination and quantification of the specific radionuclides including those known as Difficult-to-Measure Radionuclides (RDM). The analysis of the RDM's generally involves complex radiochemical analysis for purification and separation of the radionuclides, which are expensive and time-consuming. The objective of this work was to define a methodology for sequential analysis of the isotopes of uranium, neptunium, plutonium, americium and curium present in a type of radioactive waste, evaluating chemical yield, analysis of time spent, amount of secondary waste generated and cost. Three methodologies were compared and validated that employ ion exchange (TI + EC), extraction chromatography (EC) and extraction with polymers (ECP). The waste chosen was the activated charcoal from the purification system of primary circuit water cooling the reactor IEA-R1. The charcoal samples were dissolved by acid digestion followed by purification and separation of isotopes with ion exchange resins, extraction and chromatographic extraction polymers. Isotopes were analyzed on an alpha spectrometer, equipped with surface barrier detectors. The chemical yields were satisfactory for the methods TI + EC and EC. ECP method was comparable with those methods only for uranium. Statistical analysis as well the analysis of time spent, amount of secondary waste generated and cost revealed that EC method is the most effective for identifying and quantifying U, Np, Pu, Am and Cm present in charcoal. (author)

General physical fundamentals of isotope hydrology

International Nuclear Information System (INIS)

Moser, H.; Rauert, W.

1976-01-01

A description is given of the measurement and measuring units of stable isotopes, the physical properties, measurement and measuring units of radioactive isotopes, the fundamentals of the tracer technique, the environmental isotope distribution in the hydrosphere and the radiation protection in isotope hydrological investigations. (HK) [de

Canada's isotope crisis : what next?

Energy Technology Data Exchange (ETDEWEB)

Nathwani, J.; Wallace, D. (eds.)

2010-07-01

Canada urgently requires a rigorous debate on the strategic options for ensuring a robust, reliable, and affordable supply of radioactive isotopes. Should the debate be confined to how Canada can best develop the necessary technologies solely for our own use or should Canada abandon the idea of producing its own isotope supply and any future aspirations to serve the global market? Canada's Isotope Crisis focuses on the central policy question: do we dare to try to shape the future or do we retreat into silence because we are not prepared to make the necessary investments for the future well-being of Canadians? This volume showcases pointed essays and analysis from members of the academy and individuals who have made contributions to the development of medical isotopes and pioneered their use in medical practice. It also includes commentary from those involved in the production, manufacturing, processing, and distribution of isotopes. Canada's Isotope Crisis is a multi-disciplinary effort that addresses the global dimension of isotope supply and combines expert opinions on the present and past with knowledge of the relevant government agencies and the basis for their decisions at critical junctures.

Design of a positional tracking and radiological alarm system for transportation of radioactive isotopes

International Nuclear Information System (INIS)

Saindane, Shashank; Pujari, R.N.; Narsaiah, M.V.R.; Chaudhury, Probal; Pradeepkumar, K.S.

2016-01-01

The safety aspects during the transport of radioactive material have to ensure that even in event of accident the potential of radiation exposure to public is extremely small. Continuous monitoring and online data transfer to emergency control room will strengthen the emergency preparedness to response to any such accident during transport of radioactive material. The paper presents the combined application of Geographical Information Systems (GIS), Global Positioning System (GPS), General Packet Radio Service (GPRS) and the Internet for tracking the shipment vehicle transporting radioactive isotopes for use in the medical industry. The key features of the prototype system designed are realtime radiological status update along with photo snap of the shipping flask at predefined interval along with positional coordinates, GIS platform and a web-based user interface. The system consists of a GM based radiation monitoring device (RMD) along with a LAN camera, GPS for tracking the shipment vehicle, a communications server, a web-server, a database server, and a map server. The RMD and tracking device mounted in the shipment vehicle collects location and radiological information on real-time via the GPS. This information is transferred continuously through GPRS to a central database. The users will be able to view the current location of the vehicle via a web-based application

Low (50 keV) and medium (∼10 MeV) energy radioactive beams at Louvain-la-Neuve

International Nuclear Information System (INIS)

Huyse, M.; Decrock, P.; Dendooven, P.; Reusen, G.; Duppen, P. Van; Wauters, J.

1991-01-01

Low energy radioactive beams are produced at the Leuven Isotope Separator On Line (LISOL) facility in Louvain-la-Neuve. The beams are used for standard nuclear spectroscopy studies and for nuclear orientation on line measurements. Since September 1987 a new project has been started up to accelerate radioactive beams to energies in the range of astrophysical interest. A beam of 10 6 13 N ions per seconde with an energy of 8.5 MeV has been produced last June. (author) 11 refs.; 1 fig.; 1 tab

The radioactive earth

International Nuclear Information System (INIS)

Plant, J.A.; Saunders, A.D.

1996-01-01

Uranium, thorium and potassium are the main elements contributing to natural terrestrial radioactivity. The isotopes 238 U, 235 U, 232 Th and 40 K decay with half-lives so long that significant amounts remain in the earth, providing a continuing source of heat. The slow decay of these isotopes also provides the basis for radiometric age dating and isotopic modelling of the evolution of the earth and its crust. There is a complex interplay between their heat production and the processes involved in crust formation. Phenomena such as volcanism, earthquakes, and large-scale hydrothermal activity associated with ore deposition reflect the dissipation of heat energy from the earth, much of which is derived from natural radioactivity. The higher levels of radioactive elements during the early history of the earth resulted in higher heat flow. All three of the radioactive elements are strongly partitioned into the continental crust, but within the crust their distribution is determined by their different chemical properties. The behaviour of U, which has two commonly occurring oxidation states, is more complex than that of Th and K. Uranium deposits are diverse, and are mostly associated with granites, acid volcanics, or detrital sedimentary rocks. The most important U deposits economically are unconformity-type ores of Proterozoic age, in which U is enriched by up to 5 x 10 6 with respect to bulk earth values. In some cases natural radioactivity can be of environmental concern. The most significant risk is posed by accumulations of radon, the gaseous daughter product of U. (author)

Travel in the depth of radioactivity

International Nuclear Information System (INIS)

1996-09-01

This educational booklet gives a general presentation of radioactivity: origin of natural radioactivity, characteristics of atoms and isotopes, the radioactivity phenomenon, its decay and measurement units, the radiations and their use in medicine, industry, agriculture and food industry, biology etc.. (J.S.)

Intense ^31-35Ar beams produced with a nanostructured CaO target at ISOLDE

DEFF Research Database (Denmark)

Ramos, J. P.; Gottberg, A.; Mendonça, T. M.

2014-01-01

At the ISOLDE facility at CERN, thick targets are bombarded with highly energetic pulsed protons to produce radioactive ion beams (RIBs). The isotopes produced in the bulk of the material have to diffuse out of the grain and effuse throughout the porosity of the material to a transfer line which ...

Utilization of small-amount of radioactive isotope. Report of Technical Committee for Using Minor Radioactive Sources, Section of Physical Science and Industry, JRIAS. (1)

International Nuclear Information System (INIS)

1999-01-01

The report of this series is a summary of considerations made by the committee which was founded in January, 1991, for stimulating the utilization of small-amount radioactive isotopes. The present report (1) is composed of three chapters concerning the purpose above mentioned and achievement of the committee, and reasonable regulation for the sealed isotopes. For the purpose, analysis was made for the present states of small-amount radioisotope utilization and of legal regulation and proposals were done by the committee. In the past, the first (1/1, 1991-5/31, 1992) and second (6/1, 1992 5/31, 1994) terms of the committee investigated the present states of utilization and safety handling in Japan and foreign countries, methods for stimulation, education and re-evaluation of the past trials for technology of those sub-legal isotopes together with translation of IAEA SAFETY SERIES No. 104 into Japanese, which was published in the journal Radioisotopes vol.44 (1995), for reference of the present states in Japan and foreign countries. In the chapter of proposal for the reasonable regulation for the sealed isotopes, the present committee investigated the present states of utilization of the industrial instruments and daily necessities which are equipped with small-amount radioisotopes, their legal and safety problems involved and the basis of calculation of exemption level, and made proposals for reasonable regulation. (K.H.)

Thin and thick targets for radioactive ion beam production at SPIRAL1 facility

Science.gov (United States)

Jardin, P.; Bajeat, O.; Delahaye, P.; Dubois, M.; Kuchi, V.; Maunoury, L.

2018-05-01

The upgrade of the Système de Production d'Ions Radioactifs Accélérés en Ligne (SPIRAL1) facility will deliver its new Radioactive Ion Beams (RIB) by summer 2017. The goal of the upgrade is an improvement of the performances of the installation in terms of isotopes species and ion charge states [1]. Ion beams are produced using the Isotope Separator On Line Method, consisting in an association of a primary beam of stable ions, a hot target and an ion source. The primary beam impinges on the material of the target. Radioactive isotopes are produced by nuclear reactions and propagate up to the source, where they are ionized and accelerated to create a RIB. One advantage of SPIRAL1 driver is the variety of its available primary beams, from carbon to uranium with energies up to 95 MeV/A. Within the SPIRAL1 upgrade, they will be combined with targets made of a large choice of materials, extending in this way the number of possible nuclear reactions (fusion-evaporation, transfer, fragmentation) for producing a wider range of isotopes, up to regions of the nuclide chart still scarcely explored. Depending on the reaction process, on the collision energy and on the primary beam power, thin and thick targets are used. As their functions can be different, their design must cope with specific constraints which will be described. After a presentation of the goals of present and future SPIRAL1 Target Ion Source System, the main target features, studies and designs under progress are presented.

Criminal Protection of the Consumer of Irradiated food and Consumer Protection Against Contaminated Food with Radioactive Isotopes

International Nuclear Information System (INIS)

El-Baroudy, M.M.

2003-01-01

The widespread peaceful applications of atomic energy in food and agriculture had various positive and negative impacts on the economies of food and its production. Food is positively affected through either its treatment by ionizing radiation to preserve and reduce losses in it or by using mutations treated by ionizing radiation for improving their productivity. On the other hand, negative effects of nuclear energy on food are caused by nuclear explosions in nuclear weapons testing as well as by different nuclear energy applications and the wastes formed as a result of it. These activities can cause different contamination levels of the environment and particularly, the arable land. This in turn leads to the production of contaminated food with radioactive isotopes. Consequently, the present work which is subdivided into two parts, involves a study of both the positive and negative effects of ionizing radiations and radioactive isotopes on food. The first part deals with the legal protection of food treated by ionizing radiations to preserve it, explaining the related different legal and regulatory aspects. Food irradiation processes should be carried out in a framework of the national control regulations and in a way that is consistent with the reference standards adopted internationally for the safety and hygiene of food

Using MASHA+TIMEPIX Setup for Registration Beta Decay Isotopes Produced in Heavy Ion Induced Reactions

Science.gov (United States)

Rodin, A. M.; Belozerov, A. V.; Chernysheva, E. V.; Dmitriev, S. N.; Gulyaev, A. V.; Gulyaeva, A. V.; Itkis, M. G.; Novoselov, A. S.; Oganessian, Yu. Ts.; Salamatin, V. S.; Stepantsov, S. V.; Vedeneev, V. Yu.; Yukhimchuk, S. A.; Krupa, L.; Granja, C.; Pospisil, S.; Kliman, J.; Motycak, S.; Sivacek, I.

2015-06-01

Radon and mercury isotopes were produced in multi nucleon transfer (48Ca + 232Th) and complete fusion (48Ca + naturalNd) reactions, respectively. The isotopes with given masses were detected using two detectors: a multi-strip detector of the well-type (made in CANBERRA) and a position-sensitive quantum counting hybrid pixel detector of the TIMEPIX type. The isotopes implanted into the detectors then emit alpha- and betaparticles until reaching the long lived isotopes. The position of the isotopes, the tracks, the time and energy of beta-particles were measured and analyzed. A new software for the particle recognition and data analysis of experimental results was developed and used. It was shown that MASHA+ TIMEPIX setup is a powerful instrument for investigation of neutron-rich isotopes far from stability limits.

Isotopes in hydrology of ground water

International Nuclear Information System (INIS)

Rodriguez, N.; C, O.

1996-01-01

Fundamental concepts on Radioactivity, Isotopes, Radioisotopes, Law of Nuclear Decay (Middle Life concept), Radioactivity units, Types of radiation, Absorption and dispersion of both Alfa and Beta particles and both gamma and X-rays attenuation are presented. A description on Environmental Isotopes (those that are presented in natural form in the environment and those that can't be controlled by the humans), both stables and unstable (radioisotopes) isotopes is made. Isotope hydrology applications in surface water investigations as: Stream flow measurements and Atmosphere - surface waters interrelationship is described. With relation to the groundwater investigations, different applications of the isotope hydrology, its theoretical base and its methodology are presented to each one of the substrates as: Unsaturated zone (soil cape), Saturated zone (aquifer cape), Surface waters - ground waters interrelationship (infiltration and recharge) and to hydrologic balance

Precision Gamma-Ray Branching Ratios for Long-Lived Radioactive Nuclei

Energy Technology Data Exchange (ETDEWEB)

Tonchev, Anton [Lawrence Livermore National Lab. (LLNL), Livermore, CA (United States)

2017-10-19

Many properties of the high-energy-density environments in nuclear weapons tests, advanced laser-fusion experiments, the interior of stars, and other astrophysical bodies must be inferred from the resulting long-lived radioactive nuclei that are produced. These radioactive nuclei are most easily and sensitively identified by studying the characteristic gamma rays emitted during decay. Measuring a number of decays via detection of the characteristic gamma-rays emitted during the gamma-decay (the gamma-ray branching ratio) of the long-lived fission products is one of the most straightforward and reliable ways to determine the number of fissions that occurred in a nuclear weapon test. The fission products ¹⁴⁷Nd, ¹⁴⁴Ce, ¹⁵⁶Eu, and certain other long-lived isotopes play a crucial role in science-based stockpile stewardship, however, the large uncertainties (about 8%) on the branching ratios measured for these isotopes are currently limiting the usefulness of the existing data [1,2]. We performed highly accurate gamma-ray branching-ratio measurements for a group of high-atomic-number rare earth isotopes to greatly improve the precision and reliability with which the fission yield and reaction products in high-energy-density environments can be determined. We have developed techniques that take advantage of new radioactive-beam facilities, such as DOE's CARIBU located at Argonne National Laboratory, to produce radioactive samples and perform decay spectroscopy measurements. The absolute gamma-ray branching ratios for ¹⁴⁷Nd and ¹⁴⁴Ce are reduced <2% precision. In addition, high-energy monoenergetic neutron beams from the FN Tandem accelerator in TUNL at Duke University was used to produce ¹⁶⁷Tm using the ¹⁶⁹Tm(n,3n) reaction. Fourtime improved branching ratio of ¹⁶⁷Tm is used now to measure reaction-in-flight (RIF) neutrons from a burning DT capsule at NIF [10]. This represents the

The cobalt radioactive isotopes in environment; Les isotopes radioactifs du cobalt dans l'environnement

Energy Technology Data Exchange (ETDEWEB)

NONE

2007-07-01

For the year 1993 the total activity released in cobalt is 69 GBq for the whole of nuclear power plants. The part of activity in cobalt for La Hague in 1993 is 8 GBq of {sup 58}Co and 2 GBq of {sup 60}Co. The radioactive isotopes released by nuclear power plants or the reprocessing plant of La Hague under liquid effluents are shared by half between {sup 58}Co and {sup 60}Co. The exposure to sealed sources is the most important risk for the cobalt. The risk of acute exposure can associate a local irradiation of several decades of grays inducing a radiological burns, deep burn to treat in surgery by resection or graft even amputation. A global irradiation of organism for several grays induces an acute irradiation syndrome, often serious. At long term the stochastic effects are represented by leukemia and radio-induced cancers. The increase of probability of their occurrence is 1% by sievert. We must remind that the natural spontaneous probability is 25%. (N.C.)

Annual report 1984. Radioactive isotope department

International Nuclear Information System (INIS)

Muenze, R.

1985-11-01

New technologies for production and application of radionuclides and synthesis of radioactive compounds are reported. Special importance is attributed to the characterization of radioactive compounds and the quality check of /sup 99m/Tc- and 14 C-labelled complexes within animal tests. An extensive list of publications and lectures illustrates the international cooperation of research in the field of radiochemistry

Radioactively labelled vitamin B12

International Nuclear Information System (INIS)

Charlton, J.C.; Hamilton, A.L.

1978-01-01

The application concerns the manufacture of radioactive forms of vitamin B-12 in which the cobalt atom present in the vitamin B-12 molecule is replaced with a radioactive isotope of cobalt, usually cobalt-57 or cobalt-58. Such radioactive forms of B-12 are used extensively in the diagnosis of B-12 deficiency states

A new method for the labelling of proteins with radioactive arsenic isotopes

Energy Technology Data Exchange (ETDEWEB)

Jennewein, M. [Institute of Nuclear Chemistry, Johannes Gutenberg University of Mainz, Fritz-Strassmann-Weg 2, 55128 Mainz (Germany); Hermanne, A. [VUB Cyclotron, University of Brussels, Laarbeeklaan 103, 1090 Brussels (Belgium); Mason, R.P. [Department of Radiology, Advanced Radiological Sciences, University of Texas Southwestern Medical Center at Dallas, Dallas, Texas (United States); Thorpe, P.E. [Department of Pharmacology and Simmons and Hamon Cancer Centers, University of Texas Southwestern Medical Center at Dallas, Dallas, TX (United States); Roesch, F. [Institute of Nuclear Chemistry, Johannes Gutenberg University of Mainz, Fritz-Strassmann-Weg 2, 55128 Mainz (Germany)]. E-mail: frank.roesch@uni-mainz.de

2006-12-20

Radioarsenic labelled radiopharmaceuticals could be a valuable asset to positron emission tomography. In particular, the long half-lives of {sup 72}As (T{sub 1/2}=26h) and {sup 74}As (T{sub 1/2}=17.8d) allow to investigate slow physiological or metabolical processes, like the enrichment and distribution of monoclonal antibodies (mab) in tumour tissue. In this work, a new method for the labelling of proteins with various radioactive arsenic isotopes was developed. For this purpose, two proteins, namely a chimeric IgG{sub 3} monoclonal antibody, ch3G4, directed against anionic phospholipids, and Rituxan (Rituximab), were labelled as a proof of principle with no-carrier-added radioarsenic isotopes ({sup 74}As and {sup 77}As). The developed labelling chemistry gives high yields (>99.9%), is reliable and could easily be transferred to automated labelling systems in a clinical environment. At least for the mab used in this work, this route of radioarsenic labelling does not affect the immunoreactivity of the product. The arsenic label stays stable for up to 72h at the molecular mass of the monoclonal antibody, which is in particular relevant to follow the pharmacology and pharmacokinetics of the labelled mab for several days.

Isotope hydrogeological study of the underground repository for radioactive wastes at Morsleben

International Nuclear Information System (INIS)

Gellermann, R.; Hebert, D.

1991-01-01

As a contribution of safety assessment of the underground repository for radioactive wastes (ERA) in Morsleben isotope investigations in the hydrosphere has been carried out. The measured tritium concentrations of brines infiltrating into the mine cannot be interpreted in a conventional way due to contamination of mine air with tritium. However, modelling the isotope exchange allows conclusions regarding the water balance of the dripping brines. A complex interpretation which includes hydrogeochemical data results in a qualitative assessment of the infiltrating brines in regard to their hazard potential. An acute danger cannot be derived from the data available up to the present. The natural input of cosmogenic radionuclides (tritium, radiocarbon) into the aquifers above the salt level permits to study radionuclide migration at the ERA site. Tritium from the nuclear weapon tests is detectable up to a depth of 50 m below groundwater level with a maximum in about 20 m. From these data infiltration velocities of 1.6 m/a at maximum and 0.9 m/a in average are derived. The 14 C measurements of samples from more than 100 m depth yield model ages in the order of 10 4 years. This indicates a significantly reduced groundwater dynamic in the deeper horizons. (orig.) [de

Enhanced production and isotope enrichment of recombinant glycoproteins produced in cultured mammalian cells

Energy Technology Data Exchange (ETDEWEB)

Skelton, David; Goodyear, Abbey [Florida State University, Department of Chemistry and Biochemistry (United States); Ni, DaQun; Walton, Wendy J.; Rolle, Myron; Hare, Joan T. [Florida State University, Institute of Molecular Biophysics (United States); Logan, Timothy M., E-mail: tlogan@fsu.ed [Florida State University, Department of Chemistry and Biochemistry (United States)

2010-10-15

NMR studies of post-translationally modified proteins are complicated by the lack of an efficient method to produce isotope enriched recombinant proteins in cultured mammalian cells. We show that reducing the glucose concentration and substituting glutamate for glutamine in serum-free medium increased cell viability while simultaneously increasing recombinant protein yield and the enrichment of non-essential amino acids compared to culture in unmodified, serum-free medium. Adding dichloroacetate, a pyruvate dehydrogenase kinase inhibitor, further improves cell viability, recombinant protein yield, and isotope enrichment. We demonstrate the method by producing partially enriched recombinant Thy1 glycoprotein from Lec1 Chinese hamster ovary (CHO) cells using U-{sup 13}C-glucose and {sup 15}N-glutamate as labeled precursors. This study suggests that uniformly {sup 15}N,{sup 13}C-labeled recombinant proteins may be produced in cultured mammalian cells starting from a mixture of labeled essential amino acids, glucose, and glutamate.

Enhanced production and isotope enrichment of recombinant glycoproteins produced in cultured mammalian cells

International Nuclear Information System (INIS)

Skelton, David; Goodyear, Abbey; Ni, DaQun; Walton, Wendy J.; Rolle, Myron; Hare, Joan T.; Logan, Timothy M.

2010-01-01

NMR studies of post-translationally modified proteins are complicated by the lack of an efficient method to produce isotope enriched recombinant proteins in cultured mammalian cells. We show that reducing the glucose concentration and substituting glutamate for glutamine in serum-free medium increased cell viability while simultaneously increasing recombinant protein yield and the enrichment of non-essential amino acids compared to culture in unmodified, serum-free medium. Adding dichloroacetate, a pyruvate dehydrogenase kinase inhibitor, further improves cell viability, recombinant protein yield, and isotope enrichment. We demonstrate the method by producing partially enriched recombinant Thy1 glycoprotein from Lec1 Chinese hamster ovary (CHO) cells using U- 13 C-glucose and 15 N-glutamate as labeled precursors. This study suggests that uniformly 15 N, 13 C-labeled recombinant proteins may be produced in cultured mammalian cells starting from a mixture of labeled essential amino acids, glucose, and glutamate.

ICP-MS for isotope ratio measurement

Science.gov (United States)

The use of stable isotopes in mineral nutrition research has become a fundamental aspect of conducting this research. A gradual transition has occurred, now virtually complete, from radioactive isotope studies to those using stable isotopes. Although primarily used in human research, mineral stable ...

Isotope Production and Distribution Program`s Fiscal Year 1997 financial statement audit

Energy Technology Data Exchange (ETDEWEB)

NONE

1998-03-27

The Department of Energy Isotope Production and Distribution Program mission is to serve the national need for a reliable supply of isotope products and services for medicine, industry and research. The program produces and sells hundreds of stable and radioactive isotopes that are widely utilized by domestic and international customers. Isotopes are produced only where there is no U.S. private sector capability or other production capacity is insufficient to meet U.S. needs. The Department encourages private sector investment in new isotope production ventures and will sell or lease its existing facilities and inventories for commercial purposes. The Isotope Program reports to the Director of the Office of Nuclear Energy, Science and Technology. The Isotope Program operates under a revolving fund established by the Fiscal Year (FY) 1990 Energy and Water Appropriations Act and maintains financial viability by earning revenues from the sale of isotopes and services and through annual appropriations. The FY 1995 Energy and Water Appropriations Act modified predecessor acts to allow prices charged for Isotope Program products and services to be based on production costs, market value, the needs of the research community, and other factors. Although the Isotope Program functions as a business, prices set for small-volume, high-cost isotopes that are needed for research purposes may not achieve full-cost recovery. As a result, isotopes produced by the Isotope Program for research and development are priced to provide a reasonable return to the U.S. Government without discouraging their use. Commercial isotopes are sold on a cost-recovery basis. Because of its pricing structure, when selecting isotopes for production, the Isotope Program must constantly balance current isotope demand, market conditions, and societal benefits with its determination to operate at the lowest possible cost to U.S. taxpayers. Thus, this report provides a financial analysis of this situation.

The centenary of the discovery of isotopes

International Nuclear Information System (INIS)

Soulie, Edgar

2013-01-01

This article recalls works performed by different scientists (Marckwald and Keetman, Stromholm and Svedberg, Soddy, Thompson, Aston) which resulted in the observation and identification of the existence of isotopes. The author also recalls various works related to mechanisms of production of isotopes, the discovery of uranium fission and the principle of chain reaction. The author notably evokes French scientists involved in the development of mass spectroscopy and in the research and applications on isotopes within the CEA after the Second World War. A bibliography of article and books published by one of them, Etienne Roth, is provided. References deal with nuclear applications of chemical engineering (heavy water and its production, chemical processes in fission reactors, tritium extraction and enrichment), isotopic fractioning and physical-chemical processes, mass spectrometry and isotopic analysis, isotopic geochemistry (on 07;Earth, search for deuterium in moon rocks and their consequences), first dating and the Oklo phenomenon, radioactive dating, water and climate (isotopic hydrology, isotopes and hailstone formation, the atmosphere), and miscellaneous scientific fields (nuclear measurements and radioactivity, isotopic abundances and atomic weight, isotopic separation and use of steady isotopes)

Method for determination of radioactive iodine isotopes in environmental objects and biologic materials

International Nuclear Information System (INIS)

Dubynin, O.D.; Pogodin, R.I.

1981-01-01

The method proposed for determination of radioactive iodine isotopes content in environmental objects and biologic materials is based on the extraction of iodine with carbon tetrachloride and subsequent precipitation of bismuthyl iodine (BiOI) in perchloric medium. Sample preparation for analysis is carried out using conventional alkaline ashing methods. Quantitative iodine separation is hampered if macroquantities of Cl - , Br - , SO 4 2 - , SO 8 2 - , Cr 2 O 7 2 - and other ions are present in the solution. Iodine extraction is carried out before its precipitation. Separated iodine preparation activity is measured using scintillation (NaI) Tl gamma spectrometer. The method's sensitivity when measuring iodine-131 preparations makes up 0.07 Bq per 1 sample with the error +-25 %

Russian ElectroKhimPribor integrated plant - producer and supplier of enriched stable isotopes

International Nuclear Information System (INIS)

Tatarinov, A.N.; Polyakov, L.A.

1997-01-01

Russian ElectroKhimPribor Integrated Plant, as well as ORNL, is a leading production which manufactures and supplied to the world market such specific products as stable isotopes. More than 200 isotopes of 44 elements can be obtained at its electromagnetic separator. Changes being underway for a few last years in Russia affected production and distribution of stable isotopes. There arose a necessity in a new approach to handling work in this field so as to create favourable conditions for both producers and customers. As a result, positive changes in calutron operation at ElectroKhimPribor has been reached; quality management system covering all stages of production has been set up; large and attractive stock of isotopes has been created; prospective scientific isotope-based developments are taken into account when planning separation F campaigns; executing the contracts is guaranteed; business philosophy has been changed to meet maximum of customer needs. For more than forty years ElectroKhimPribor have had no claim from customers as to quality of products or implementing contracts. Supplying enriched stable isotopes virtually to all the world's leading customers, ElectroKhimPribor cooperates successfully with Canadian company Trace Science since 1996

An isotopic analysis process with optical emission spectrometry on a laser-produced plasma

International Nuclear Information System (INIS)

Mauchien, P.; Pietsch, W.; Petit, A.; Briand, A.

1994-01-01

The sample that is to be analyzed is irradiated with a laser beam to produce a plasma at the sample surface; the spectrum of the light emitted by the plasma is analyzed and the isotope composition of the sample is derived from the spectrometry. The process is preferentially applied to uranium and plutonium; it is rapid, simpler and cheaper than previous methods, and may be applied to 'in-situ' isotopic analysis in nuclear industry. 2 figs

Determination of stable and radioactive isotopes in rain water in Sahel in 1975 and 1976

International Nuclear Information System (INIS)

Baudet, J.; Abi, B.

1979-01-01

The problem of desertification in Africa incites to materialize the circuit of the water vapour between its main source, the Gulf of Guinea, and its precipitation site. Some rainwater samples have been collected in Ouagadougou in 1975 and 1976 during the rainy season. The dosage of the stable isotopes D and O 18 and radioactive isotope T shows that in 1975, a year with a general rain deficit, the rain was formed in a continental air mass. On the contrary, in 1976, a year with excess rain, the rain was formed in a maritime air mass. A study of the wind flows at 600, 900, 1500 and 2100 m shows that in 1975 the monsoon penetration is limited to the bottom of the Gulf of Guinea facing Cameroons, while in 1976 it entered the African Continent through the whole Gulf Coast, from Senegal to Cameroons. In 1976, the monsoon went up in latitude 3 0 to 5 0 more to the north than in 1975 [fr

Particle transfer spectroscopy using radioactive targets

CERN Document Server

Naumann, R A

1976-01-01

The practicality of general use of radioactive targets to study nuclei off the stability line by transfer spectroscopy is examined. Some advantages of this spectroscopic technique are illustrated with recent results from (p, t) and (t, p) stable target studies of negative parity core-coupled states systematically occurring in 4 adjacent odd silver isotopes. Preliminary results from the study of the /sup 205/Pb (t, p)/sup 207/Pb reaction using reactor produced 3*10/sup 7/ year lead 205 are given. (3 refs).

Radioactive isotope production for medical applications using Kharkov electron driven subcritical assembly facility

International Nuclear Information System (INIS)

Talamo, A.; Gohar, Y.

2007-01-01

Kharkov Institute of Physics and Technology (KIPT) of Ukraine has a plan to construct an accelerator driven subcritical assembly. The main functions of the subcritical assembly are the medical isotope production, neutron thereby, and the support of the Ukraine nuclear industry. Reactor physics experiments and material research will be carried out using the capabilities of this facility. The United States of America and Ukraine have started collaboration activity for developing a conceptual design for this facility with low enrichment uranium (LEU) fuel. Different conceptual designs are being developed based on the facility mission and the engineering requirements including nuclear physics, neutronics, heat transfer, thermal hydraulics, structure, and material issues. Different fuel designs with LEU and reflector materials are considered in the design process. Safety, reliability, and environmental considerations are included in the facility conceptual design. The facility is configured to accommodate future design improvements and upgrades. This report is a part of the Argonne National Laboratory Activity within this collaboration for developing and characterizing the subcritical assembly conceptual design. In this study, the medical isotope production function of the Kharkov facility is defined. First, a review was carried out to identify the medical isotopes and its medical use. Then a preliminary assessment was performed without including the self-shielding effect of the irradiated samples. Finally, more detailed investigation was carried out including the self-shielding effect, which defined the sample size and irradiation location for producing each medical isotope. In the first part, the reaction rates were calculated as the multiplication of the cross section with the unperturbed neutron flux of the facility. Over fifty isotopes were considered and all transmutation channels are used including (n,γ), (n,2n), (n,p), and (γ,n). In the second part, the parent

Radioactive isotope production for medical applications using Kharkov electron driven subcritical assembly facility.

Energy Technology Data Exchange (ETDEWEB)

Talamo, A.; Gohar, Y.; Nuclear Engineering Division

2007-05-15

Kharkov Institute of Physics and Technology (KIPT) of Ukraine has a plan to construct an accelerator driven subcritical assembly. The main functions of the subcritical assembly are the medical isotope production, neutron thereby, and the support of the Ukraine nuclear industry. Reactor physics experiments and material research will be carried out using the capabilities of this facility. The United States of America and Ukraine have started collaboration activity for developing a conceptual design for this facility with low enrichment uranium (LEU) fuel. Different conceptual designs are being developed based on the facility mission and the engineering requirements including nuclear physics, neutronics, heat transfer, thermal hydraulics, structure, and material issues. Different fuel designs with LEU and reflector materials are considered in the design process. Safety, reliability, and environmental considerations are included in the facility conceptual design. The facility is configured to accommodate future design improvements and upgrades. This report is a part of the Argonne National Laboratory Activity within this collaboration for developing and characterizing the subcritical assembly conceptual design. In this study, the medical isotope production function of the Kharkov facility is defined. First, a review was carried out to identify the medical isotopes and its medical use. Then a preliminary assessment was performed without including the self-shielding effect of the irradiated samples. Finally, more detailed investigation was carried out including the self-shielding effect, which defined the sample size and irradiation location for producing each medical isotope. In the first part, the reaction rates were calculated as the multiplication of the cross section with the unperturbed neutron flux of the facility. Over fifty isotopes were considered and all transmutation channels are used including (n,{gamma}), (n,2n), (n,p), and ({gamma},n). In the second part

Laser spectroscopy of neutron deficient gold and platinum isotopes

International Nuclear Information System (INIS)

Savard, G.

1988-03-01

A new method for on-line laser spectroscopy of radioactive atoms based on the resonant ionization spectroscopy of laser-desorbed radioactive samples has been devised. An experimental setup has been installed on-line at the ISOCELE mass separator in Orsay (France) and experiments have been performed on the region of transitional nuclei around Z=79. Isotopic shift measurements on four new isotopes 194 Au, 196 Au, 198 Au, 199 Au have been performed on gold and results on the neutron deficient isotopes down to 186 Au have been obtained confirming the nuclear ground-state shape transition from oblate to prolate between 187 Au and 186 Au. The first isotopic shift measurements on radioactive platinum isotopes have been obtained on 186 Pt, 188 Pt, 189 Pt. Indications of a shape transition have been observed between 186 Pt and 188 Pt. The extracted experimental changes in mean square charge radii δ 2 > A,A' along isotopic chains are compared to self-consistent Hartree-Fock plus BCS calculations

Table of nuclear reactions and subsequent radioactive dacays induced by 14-MeV neutrons

International Nuclear Information System (INIS)

Tsukada, Kineo

1977-09-01

Compilation of the data on nuclear reactions and subsequent radioactive decays induced by 14-MeV neutrons is presented in tabular form for most of the isotopes available in nature and for some of the artificially-produced isotopes, including the following items: Nuclide (isotopic abundance), type of nuclear reaction, reaction Q-value, reaction product, type of decay, decay Q-value, half-life of reaction product, decay product, maximum reaction cross section, neutron energy for maximum cross section, reaction cross section for 14 MeV neutrons, saturated radioactivity induced by irradiation of a neutron flux of 1 n/cm 2 sec for a mol of atoms, and reference for the cross section. The mass number dependence of (n, γ), (n, 2n), (n, p), (n, d), (n, t), (n, 3 He) and (n, α) reaction cross sections for 14-MeV neutrons is given in figures to show general trends of the cross sections

The oxygen isotope composition of earth's oldest rocks and evidence of a terrestrial magma ocean

DEFF Research Database (Denmark)

Rumble, D.; Bowring, S.; Iizuka, T.

2013-01-01

Analysis of Hadean and Archean rocks for O-16-O-17-O-18 isotopes demonstrates that the Terrestrial Mass Fractionation Line of oxygen isotopes has had the same slope and intercept for at least the past 4.0 and probably for as long as 4.2Ga. The homogenization of oxygen isotopes required to produce....... But other sources of heat for global melting cannot be excluded such as bolide impacts during early accretion of proto-Earth, the decay of short-lived radioactive isotopes, or the energy released during segregation of core from mantle.......Analysis of Hadean and Archean rocks for O-16-O-17-O-18 isotopes demonstrates that the Terrestrial Mass Fractionation Line of oxygen isotopes has had the same slope and intercept for at least the past 4.0 and probably for as long as 4.2Ga. The homogenization of oxygen isotopes required to produce...... such long-lived consistency was most easily established by mixing in a terrestrial magma ocean. The measured identical oxygen isotope mass fractionation lines for Earth and Moon suggest that oxygen isotope reservoirs of both bodies were homogenized at the same time during a giant moon-forming impact...

Radioactivity and the French uranium bearing minerals

International Nuclear Information System (INIS)

Guiollard, P.Ch.; Boisson, J.M.; Leydet, J.C.; Meisser, N.

1998-01-01

This special issue of Regne Mineral journal is entirely devoted to the French uranium mining industry. It comprises 4 parts dealing with: the uranium mining industry in France (history, uranium rush, deposits, geologic setting, prosperity and recession, situation in 1998, ore processing); radioactivity and the uranium and its descendants (discovery, first French uranium bearing ores, discovery of radioactivity, radium and other uranium descendants, radium mines, uranium mines, atoms, elements and isotopes, uranium genesis, uranium decay, isotopes in an uranium ore, spontaneous fission, selective migration of radionuclides, radon in mines and houses, radioactivity units, radioprotection standards, new standards and controversies, natural and artificial radioactivity, hazards linked with the handling and collecting of uranium ores, conformability with radioprotection standards, radioactivity of natural uranium minerals); the French uranium bearing minerals (composition, crystal structure, reference, etymology, fluorescence). (J.S.)

Nuclear moments and charge radii of magnesium isotopes from N=8 up to (and beyond) N=20

CERN Multimedia

Mattolat, C F; Mallion, S N; Himpe, P

2002-01-01

We propose to measure the nuclear monopole, dipole and quadrupole moments of magnesium isotopes from the neutron deficient nuclei near the N=8 shell closure ($^{21}$Mg), up to the neutron rich Mg nuclei beyond N=20 ($^{33}$Mg). The physics issues that will be addressed in this project are related to: \\begin{itemize} \\item The properties of mirror nuclei (e.g. $^{21}$Mg - $^{21}$F being members of a T=3/2 multiplet) \\item The evolution of shell structure and deformation with isospin. \\item Changes in the shell structure in the "island of inversion" around $^{32}$Mg and along the N=9 isotones. \\end{itemize} Radioactive beams of Mg isotopes will be produced by the RILlS ion source. The Mg isotopes will be resonantly polarized at the COLLAPS set-up. With $\\beta$-NMR techniques, precision measurements of g-factors and quadrupole moments of the radioactive $^{21,23}$Mg and $^{29,31,33}$Mg isotopes will be performed. Isotope shifts, thus changes in mean square charge radii, will be deduced from hyperfine spectra mea...

Evaluation of Radioactivity in Dusty Storm

International Nuclear Information System (INIS)

Mohammed, A.S; Majeed, N. A.; Nasaer, M.H.; Hoshi, H.; Abood, M.

2013-01-01

sample had been collected from the powder of the dusty storms which had been moved over Baghdad for a different months of a year 2011 by using metal containers that had manufactured locally and had been mounted over the roof of houses in particular regions of Baghdad (Kerkh and Risafa).The radioactive concentration of dust samples had been measured and analyzed by using the Gamma Spectroscopy analyzing System which consist of high purity Germanium detector of efficiency of 40 %, resolution 2keV at 1.332 MeV (Co-60) , DSA 2000 system which protective barrier made in Canberra Company , the developed Genie 2000Program and using personal computer. The measurement system for energy calibration and efficiency had been calibrated by using a standard point sources and standard source of a multi energy made by the American Canberra company. The Marnelli geometrical shape had been used to measure the activity of the samples. Results indicated the existence of the natural radioactive isotopes such as K-40, Be-7 which has been composed of as a result of the nuclear reaction between the Cosmic ray and some other elements of the atmosphere like Oxygen and Nitrogen besides the existence of radioactive isotopes which belongs to the natural Uranium series and the natural Thorium series. Highest measurements indicated the existence of industrial radioactive isotope Cs-137.The highest value of concentration for Be-7 was (381.5 Bq/kg) at Al-Shaab region, and the highest value of concentration for K-40 was (467.7 Bq/kg) and some other radioactive isotopes which belong to the series of U-238 as follows:- Bi -214 (32.6 Bq/kg), Pb-214 (33.6 Bq/kg), and radioactive isotopes which belong to the series Th-232 as follows:- Bi-212(18.6Bq/kg), Pb-212 (18.8Bq/kg),Ac-228 (30.3 Bq/kg),the highest value of concentration for the industrial Cs-137 was (26,8 Bq/kg) it was at Al-shaab region ,and this concentration is relatively high in comparison to the levels of normal concentration which exist in

Nuclear astrophysics with radioactive beams: a TRIUMF perspective

International Nuclear Information System (INIS)

Shotter, A.C.

2003-01-01

Explosive nuclear burning in stellar environments involves reactions with a wide range of isotopes. For isotopes that are unstable, information on relevant reaction rates can only generally be obtained at radioactive beam facilities. The ISAC facility at TRIUMF is purpose built to provide a wide range of radioactive beams for nuclear astrophysics purposes as well as a range of other science

Radioactivity of the soil in Vojvodina (northern province of Serbia and Montenegro).

Science.gov (United States)

Bikit, I; Slivka, J; Conkić, Lj; Krmar, M; Vesković, M; Zikić-Todorović, N; Varga, E; Curcić, S; Mrdja, D

2005-01-01

The widespread public belief that during the bombardment of Vojvodina (Yugoslavia) this region was contaminated by depleted uranium has recently raised public concern with respect to the potential contamination of agricultural products due to soil radioactivity. Based on the gamma-spectrometric analysis of 50 soil samples taken from the region of Vojvodina we concluded that there is no increase of radioactivity that could endanger the food production. Taking into account the transfer factors of 137Cs to plants, the measured activity concentrations of this isotope should not endanger the health safety of the produced food. No traces of depleted uranium have been found. The natural radioactivity levels are compared with the results form other countries.

Radioactivity of the soil in Vojvodina (northern province of Serbia and Montenegro)

International Nuclear Information System (INIS)

Bikit, I.; Slivka, J.; Conkic, Lj.; Krmar, M.; Veskovic, M.; Zikic-Todorovic, N.; Varga, E.; Curcic, S.; Mrdja, D.

2004-01-01

The widespread public belief that during the bombardment of Vojvodina (Yugoslavia) this region was contaminated by depleted uranium has recently raised public concern with respect to the potential contamination of agricultural products due to soil radioactivity. Based on the gamma-spectrometric analysis of 50 soil samples taken from the region of Vojvodina we concluded that there is no increase of radioactivity that could endanger the food production. Taking into account the transfer factors of 137 Cs to plants, the measured activity concentrations of this isotope should not endanger the health safety of the produced food. No traces of depleted uranium have been found. The natural radioactivity levels are compared with the results form other countries

Installation of an isotope separator in Debrecen

International Nuclear Information System (INIS)

Gacsi, Z.; Gulyas, J.; Vitez, A.; Csige, L.; Krasznahorkay, A.

2005-01-01

Complete text of publication follows. An isotope separator named OSIRIS was decommissioned in Studsvik, Sweden last July. Researchers there offered this equipment to us for dismantling and moving it over to ATOMKI in Debrecen for installation at the cyclotron lab and save and use it in nuclear physics and other sciences where stable and radioactive isotopes are used extensively for fundamental and applied research. Since the separator was used to separate radioactive isotopes, the ion source with its beam extracting, shaping, and transporting accessories, as well as the lining inside the bending magnet, furthermore the beam diagnostic and shaping elements in the 'switchyard' part of the separator had to stay in Studsvik because of the high radioactive contamination. In order to operate this equipment, first we have to design and manufacture these parts together with a new endstation for the collection and handling of the separated isotopes. Parallel with the installation, we also concentrate on different applications of an isotope separator, including separation of stable isotopes for labelling special compounds used in many branches of sciences, medical care, and industry, and on studying single ion implantation possibilities, as well as on the production of special targets for nuclear physics research. First we want to separate stable isotopes, and then, when we overcome all technical pitfalls, we will consider using this equipment to separate radioactive isotopes as well. Our intention is to have this equipment available to anyone at ATOMKI and elsewhere interested in using its capabilities in their own research fields. Consequently, all comments, suggestion, and ideas are welcome now and continuously, since the design and manufacture of parts can then be oriented by taking into account all the suggestions as much as possible. (author)

Efigie: a computer program for calculating end-isotope accumulation by neutron irradiation and radioactive decay

International Nuclear Information System (INIS)

Ropero, M.

1978-01-01

Efigie is a program written in Fortran V which can calculate the concentration of radionuclides produced by neutron irradiation of a target made of either a single isotope or several isotopes. The program includes optimization criteria that can be applied when the goal is the production of a single nuclide. The effect of a cooling time before chemical processing of the target is also accounted for.(author) [es

Storage of solid and liquid radioactive material

International Nuclear Information System (INIS)

Matijasic, A.; Gacinovic, O.

1961-01-01

Solid radioactive waste collected during 1961 from the laboratories of the Institute amounted to 22.5 m 3 . This report contains data about activity of the waste collected from january to November 1961. About 70% of the waste are short lived radioactive material. Material was packed in metal barrels and stored in the radioactive storage in the Institute. There was no contamination of the personnel involved in these actions. Liquid radioactive wastes come from the Isotope production laboratory, laboratories using tracer techniques, reactor cooling; decontamination of the equipment. Liquid wastes from isotope production were collected in plastic bottles and stored. Waste water from the RA reactor were collected in special containers. After activity measurements this water was released into the sewage system since no activity was found. Table containing data on quantities and activity of radioactive effluents is included in this report

Short-lived radionuclide production capability at the Brookhaven Linac Isotope Producer

International Nuclear Information System (INIS)

Mausner, L.F.; Richards, P.

1985-01-01

The Brookhaven National Linac Isotope Producer is the first facility to demonstrate the capability of a large linear accelerator for efficient and economical production of difficult-to-make, medically useful radionuclides. The linac provides a beam of 200-MeV protons at an integrated beam current of up to 60 μA. The 200-MeV proton energy is very suitable for isotope production because the spallation process can create radionuclides unavailable at lower energy accelerators or reactors. Several medically important short-lived radionuclides are presently being prepared for on-site and off-site collaborative research programs. These are iodine-123, iron-52, manganese-52m, ruthenium-97, and the rubidium-81-krypton-81m system. The production parameters for these are summarized

Tests of intestinal absorption using carbon-14-labeled isotopes

International Nuclear Information System (INIS)

Fromm, H.; Sarva, R.P.

1983-01-01

Beta radiation-emitting isotopes are being used increasingly in diagnostic gastroenterology for the study of absorption. The major reason for the popularity of radioisotopes is that their use is convenient for patient and physician alike. They often obviate naso- or orointestinal intubation and the collection, storage, and analysis of stool. The radioactivity used for the studies of digestive and absorptive processes is small and is not hazardous. In spite of the safety of the radiolabeled compounds, their use is restricted in children and pregnant women. Therefore, for most tests, promising alternative methods that make use of the stable isotope of carbon, /sup 13/C, instead of the radioactive /sup 14/C have been developed. The analysis of stable isotopes requires more sophisticated technology than that of radioactive compounds, however. Only a few centers presently are equipped and staffed to analyze stable isotopes on a routine basis. In contrast, the analysis of radioactive isotopes has become a routine procedure in almost ever major laboratory. The last decade has brought the development of several radioactive absorption tests. The clinically most useful tests relate to the study of bile acid, fat, lactose, and xylose absorption. All of these tests utilize the excretion rate of /sup 14/CO/sub 2/ in breath after ingestion of a /sup 14/C-labeled compound as a measure of the rate of its absorption or malabsorption

Regulation of naturally occurring and accelerator-produced radioactive materials. A Task Force review

International Nuclear Information System (INIS)

Nussbaumer, D.A.; Lubenau, J.O.; Cool, W.S.; Cunningham, L.J.; Mapes, J.R.; Schwartz, S.A.; Smith, D.A.

1977-06-01

The use of accelerator-produced radioisotopes (NARM), particularly in medicine, is growing rapidly. One NARM radioisotope, 226 Ra, is one of the most hazardous of radioactive materials, and 226 Ra is used by about 1 / 5 of all radioactive material users. Also, there are about 85,000 medical treatments using 226 Ra each year. All of the 25 Agreement States and 5 non-Agreement States have licensing programs covering NARM users. The Agreement States' programs for regulating NARM are comparable to their programs for regulating byproduct, source, and special nuclear materials under agreements with NRC. But there are 7 states who exercise no regulatory control over NARM users, and the remaining States have control programs which are variable in scope. There are no national, uniformly applied programs to regulate the design, fabrication and quality of sources and devices containing NARM or consumer products containing NARM which are distributed in interstate commerce. Naturally occurring radioactive material (except source material) associated with the nuclear fuel cycle is only partially subject to NRC regulation, i.e., when it is associated with source or special nuclear material being used under an active NRC license. The Task Force recommends that the NRC seek legislative authority to regulate naturally occurring and accelerator-produced radioactive materials for the reason that these materials present significant radiation exposure potential and present controls are fragmentary and non-uniform at both the State and Federal level

Production of beta-gamma coincidence spectra of individual radioxenon isotopes for improved analysis of nuclear explosion monitoring data

Science.gov (United States)

Haas, Derek Anderson

Radioactive xenon gas is a fission product released in the detonation of nuclear devices that can be detected in atmospheric samples far from the detonation site. In order to improve the capabilities of radioxenon detection systems, this work produces beta-gamma coincidence spectra of individual isotopes of radioxenon. Previous methods of radioxenon production consisted of the removal of mixed isotope samples of radioxenon gas released from fission of contained fissile materials such as 235U. In order to produce individual samples of the gas, isotopically enriched stable xenon gas is irradiated with neutrons. The detection of the individual isotopes is also modeled using Monte Carlo simulations to produce spectra. The experiment shows that samples of 131mXe, 133 Xe, and 135Xe with a purity greater than 99% can be produced, and that a sample of 133mXe can be produced with a relatively low amount of 133Xe background. These spectra are compared to models and used as essential library data for the Spectral Deconvolution Analysis Tool (SDAT) to analyze atmospheric samples of radioxenon for evidence of nuclear events.

Isotopes in environmental research

International Nuclear Information System (INIS)

Bowen, G.; Rozanski, K.; Vose, P.

1990-01-01

Radioactive and stable isotopes have long been considered a very efficient tool for studying physical and biological aspects of how the global ecosystem functions. Their applications in environmental research are numerous, embracing research at all levels. This article looks at only a few of the approaches to environmental problems that involve the use of isotopes. Special attention is given to studies of the Amazon Basin. Environmental isotopes are very efficient tools in water cycle studies. Tritium, a radioactive tracer, is especially useful in studying dynamics of water movement in different compartments of the hydrosphere, both on the local and global scales. Heavy stable isotopes of hydrogen and oxygen (deuterium and oxygen-18) provide information about steady-state characteristics of the water cycle. Isotope methods, some relatively new, have a major role in site-specific studies. Some indicative examples include: Studying turnover of organic matter. Changes in the carbon-13/carbon-12 isotopic ratio of organic matter were used to determine the respective contributions of organic carbon derived from forest and pasture. Studying biological nitrogen fixation. One of the ways nitrogen levels in soil can be maintained for productivity is by biological nitrogen fixation. Studying nitrogen availability and losses. The experimental use of nitrogen-15 is invaluable for defining losses of soil nitrogen to the atmosphere and to groundwater. Studies can similarly be done with stable and radioactive sulphur isotopes. This article indicates some potential uses of isotopes in environmental research. While the major problem of global climate change has not been specifically addressed here, the clearing of the Amazon forest, one focus of the IAEA's environmental programme, may have serious consequences for the global climate. These include substantial reduction of the amount of latent heat transported to the regions outside the tropics and acceleration of the greenhouse

The strategy and practice of radioactive waste management in the Pacific Basin

International Nuclear Information System (INIS)

Norman, N.; Gray, B.R.

1992-01-01

Radioactive waste management is an integral part of the planning process for the nuclear industry in Pacific Basin countries. This paper reviews areas of common interest and cooperation, sources of waste and current inventories, production rates, and future plans. Each level of radioactive waste requires different methods for handling, storage, and disposal. Definitions may vary In detail from country to country, but generally high level wastes are defined as those deriving from spent fuel and from reprocessing of fuel. These wastes contain transuranic elements and fission products that are highly radioactive, heat-generating and long-lived. Intermediate level and low level wastes may include, respectively, material from fuel fabrication and power generation other than spent fuel, and those wastes produced by research institutions, hospitals, and in other non-power producing Industrial uses of radioisotopes. The energy requirements of most countries are likely to continue to grow, and the use of radioactive isotopes in medicine and other non-energy industrial sectors is also expanding. The Pacific Nuclear Council member states participating in the Waste Management Working Group, are predicting, therefore, that the volume of radioactive waste for disposal will continue to grow

Accurate hydrocarbon estimates attained with radioactive isotope

International Nuclear Information System (INIS)

Hubbard, G.

1983-01-01

To make accurate economic evaluations of new discoveries, an oil company needs to know how much gas and oil a reservoir contains. The porous rocks of these reservoirs are not completely filled with gas or oil, but contain a mixture of gas, oil and water. It is extremely important to know what volume percentage of this water--called connate water--is contained in the reservoir rock. The percentage of connate water can be calculated from electrical resistivity measurements made downhole. The accuracy of this method can be improved if a pure sample of connate water can be analyzed or if the chemistry of the water can be determined by conventional logging methods. Because of the similarity of the mud filtrate--the water in a water-based drilling fluid--and the connate water, this is not always possible. If the oil company cannot distinguish between connate water and mud filtrate, its oil-in-place calculations could be incorrect by ten percent or more. It is clear that unless an oil company can be sure that a sample of connate water is pure, or at the very least knows exactly how much mud filtrate it contains, its assessment of the reservoir's water content--and consequently its oil or gas content--will be distorted. The oil companies have opted for the Repeat Formation Tester (RFT) method. Label the drilling fluid with small doses of tritium--a radioactive isotope of hydrogen--and it will be easy to detect and quantify in the sample

Nuclides and isotopes. Twelfth edition

International Nuclear Information System (INIS)

Anon.

1977-01-01

This explanatory booklet was designed to be used with the Chart of the Nuclides. It contains a brief history of the atomic theory of matter: ancient speculations, periodic properties of elements (Mendeleev table), radioactivity, early models of atomic structure, the Bohr atom, quantum numbers, nature of isotopes, artificial radioactivity, and neutron fission. Information on the pre-Fermi (natural) nuclear reactor at Oklo and the search for superheavy elements is given. The booklet also discusses information presented on the Chart and its coding: stable nuclides, metastable states, data display and color, isotopic abundances, neutron cross sections, spins and parities, fission yields, half-life variability, radioisotope power and production data, radioactive decay chains, and elements without names. The Periodic Table of the Elements is appended. 3 figures, 3 tables

Germanium detectors and natural radioactivity in food

Energy Technology Data Exchange (ETDEWEB)

Garbini, Lucia [Max-Planck-Institut fuer Physik, Muenchen (Germany); Collaboration: GeDet-Collaboration

2013-07-01

Potassium is a very important mineral for many physiological processes, like fluid balance, protein synthesis and signal transmission in nerves. Many aliments like raisins, bananas or chocolate contain potassium. Natural potassium contains 0.012% of the radioactive isotope Potassium 40. This isotope decays via β{sup +} decay into a metastable state of Argon 40, which reaches its ground state emitting a gamma of 1460 keV. A commercially produced Germanium detector has been used to measure the energy spectra of different selected food samples. It was calibrated with KCl and potassium contents were extracted. Results verify the high potassium content of commonly recommended food samples. However, the measurement quantitatively differ from the expectations in several cases. One of the most interesting results concerns chocolate bars with different percentages of cacao.

The management of radioactive wastes from small producers; La gestion des dechets radioactifs des petits producteurs

Energy Technology Data Exchange (ETDEWEB)

NONE

1996-01-01

Medicine, research and industry generate various type of radioactive wastes which have to be managed by the ANDRA, the French agency for the management of radioactive wastes. This educative booklet explains the missions of the ANDRA with respect to these small producers: collection, selection, conditioning, control and storage of wastes. (J.S.)

Future trends in the application of isotopes and radiation

Energy Technology Data Exchange (ETDEWEB)

Glubrecht, H [Institut fuer Biophysik, Technische Universitaet Hannover (Germany)

1977-12-15

Expected trends for the development of new methods and different applications of isotopes in agriculture, medicine and industrial production are discussed. In agriculture stable-isotope-labelled compounds can also be applied in field studies on the fate and metabolic processes of pesticide residues, as well as in long-lasting experiments on animal nutrition. Radioactive isotopes will continue to play a predominant role in trace element investigations, especially studies on the interaction and synergism of various trace elements in soil, plants and animals. The use of radioactive-labelled substrates and reagents will also become indispensable in enzyme research. Of the many other applications of isotopes in agriculture which might develop further, one item should be mentioned: the importance of non-radioactive labelling in ecology. Two areas of radiation application in agriculture may expect some progress from the use of neutron irradiation instead of gamma rays: plant breeding and the sterile insect technique (SIT). The advantage of sterilizing male insects by neutrons instead of gamma rays has become apparent with tsetse flies, which suffer less physiological harm when exposed to moderate neutron doses and, though sterile, remain fully competitive with wild tsetse fly males. There are also considerable further developments to be expected in the medical field. In vivo radionuclide imaging, if done by scanning, can only inform on local distribution of a radioactive-labelled pharmaceutical. Dynamic studies of function and physiologic processes have to be performed by using gamma-cameras which combine spatial localization with time variation. Short-lived radioisotopes, including cyclotron-produced positron emitters, are becoming more available, and the list of industrially manufactured radiopharmaceuticals is increasing. A most important development is tomography with positron emitters using annihilation gamma radiation. One of the most successful methods in clinical

Vietnam Project For Production Of Radioactive Beam Based On ISOL Technique With The Dalat Reactor

International Nuclear Information System (INIS)

Le Hong Khiem; Phan Viet Cuong; Fadi Ibrahim

2011-01-01

The presence in Vietnam of Dalat nuclear reactor dedicated to fundamental studies is a unique opportunity to produce Radioactive Ion (RI) Beams with the fission of a 235 U induced by the thermal neutrons produced by the reactor. We propose to produce RI beams at the Dalat nuclear reactor using ISOL (Isotope Separation On-Line) technique. This project should be a unique opportunity for Vietnamese nuclear physics community to use its own facilities to produce RI beams for studying nuclear physics at an international level. (author)

Laser Isotope Enrichment for Medical and Industrial Applications

Energy Technology Data Exchange (ETDEWEB)

Leonard Bond

2006-07-01

Laser Isotope Enrichment for Medical and Industrial Applications by Jeff Eerkens (University of Missouri), Jay Kunze (Idaho State University), and Leonard Bond (Idaho National Laboratory) The principal isotope enrichment business in the world is the enrichment of uranium for commercial power reactor fuels. However, there are a number of other needs for separated isotopes. Some examples are: 1) Pure isotopic targets for irradiation to produce medical radioisotopes. 2) Pure isotopes for semiconductors. 3) Low neutron capture isotopes for various uses in nuclear reactors. 4) Isotopes for industrial tracer/identification applications. Examples of interest to medicine are targets to produce radio-isotopes such as S-33, Mo-98, Mo-100, W-186, Sn-112; while for MRI diagnostics, the non-radioactive Xe-129 isotope is wanted. For super-semiconductor applications some desired industrial isotopes are Si-28, Ga-69, Ge-74, Se-80, Te-128, etc. An example of a low cross section isotope for use in reactors is Zn-68 as a corrosion inhibitor material in nuclear reactor primary systems. Neutron activation of Ar isotopes is of interest in industrial tracer and diagnostic applications (e.g. oil-logging). . In the past few years there has been a sufficient supply of isotopes in common demand, because of huge Russian stockpiles produced with old electromagnetic and centrifuge separators previously used for uranium enrichment. Production of specialized isotopes in the USA has been largely accomplished using old ”calutrons” (electromagnetic separators) at Oak Ridge National Laboratory. These methods of separating isotopes are rather energy inefficient. Use of lasers for isotope separation has been considered for many decades. None of the proposed methods have attained sufficient proof of principal status to be economically attractive to pursue commercially. Some of the authors have succeeded in separating sulfur isotopes using a rather new and different method, known as condensation

Laser Isotope Enrichment for Medical and Industrial Applications

International Nuclear Information System (INIS)

Leonard Bond

2006-01-01

Laser Isotope Enrichment for Medical and Industrial Applications by Jeff Eerkens (University of Missouri), Jay Kunze (Idaho State University), and Leonard Bond (Idaho National Laboratory) The principal isotope enrichment business in the world is the enrichment of uranium for commercial power reactor fuels. However, there are a number of other needs for separated isotopes. Some examples are: (1) Pure isotopic targets for irradiation to produce medical radioisotopes. (2) Pure isotopes for semiconductors. (3) Low neutron capture isotopes for various uses in nuclear reactors. (4) Isotopes for industrial tracer/identification applications. Examples of interest to medicine are targets to produce radio-isotopes such as S-33, Mo-98, Mo-100, W-186, Sn-112; while for MRI diagnostics, the non-radioactive Xe-129 isotope is wanted. For super-semiconductor applications some desired industrial isotopes are Si-28, Ga-69, Ge-74, Se-80, Te-128, etc. An example of a low cross section isotope for use in reactors is Zn-68 as a corrosion inhibitor material in nuclear reactor primary systems. Neutron activation of Ar isotopes is of interest in industrial tracer and diagnostic applications (e.g. oil-logging). . In the past few years there has been a sufficient supply of isotopes in common demand, because of huge Russian stockpiles produced with old electromagnetic and centrifuge separators previously used for uranium enrichment. Production of specialized isotopes in the USA has been largely accomplished using old ''calutrons'' (electromagnetic separators) at Oak Ridge National Laboratory. These methods of separating isotopes are rather energy inefficient. Use of lasers for isotope separation has been considered for many decades. None of the proposed methods have attained sufficient proof of principal status to be economically attractive to pursue commercially. Some of the authors have succeeded in separating sulfur isotopes using a rather new and different method, known as condensation

The possible transmutation of radioactive waste from nuclear reactors

International Nuclear Information System (INIS)

Harries, J.R.

1974-01-01

A nuclear reactor power program produces high level and long lived radioactive wastes. The high level activity is associated with fission products, but beyond 400 years the principal waste hazard is from transuranic elements produced in the reactor. Several schemes have been proposed for the transmutation of the problem isotopes into more easily handled isotopes. The neutron flux in a thermal reactor is not high enough to significantly reduce the longer lived fission product isotopes 90 Sr and 132 Gs, but the transuranic elements can be reduced by recycling through power reactors. The limitation on recycling of the transuranic elements is the separation process to remove trace quantities from the waste stream. In fast reactors the transuranic elements are the principal fuel and fast reactor waste contains only half as much 90 Sr as thermal reactors. However, the overall waste hazard is similar to thermal reactors. A sufficiently intense neutron flux for fission product transmutation could perhaps be produced by a spallation reactor driven by a proton linear accelerator or a controlled thermonuclear reactor. However, both concepts are still some years in the future. Transmutation by accelerator sources of protons, electrons of gammas tend to require more energy than neutron transmutation. (author)

Radioactive Iodine (I-131) Therapy for Hyperthyroidism

Science.gov (United States)

... Physician Resources Professions Site Index A-Z Radioactive Iodine (I-131) Therapy Radioiodine therapy is a nuclear ... thyroid cancer. When a small dose of radioactive iodine I-131 (an isotope of iodine that emits ...

Overview of linac applications at future radioactive beam facilities

International Nuclear Information System (INIS)

Nolen, J.A.

1996-01-01

There is considerable interest worldwide in the research which could be done at a next generation, advanced radioactive beam facility. To generate high quality, intense beams of accelerated radionuclides via the open-quotes isotope separator on-lineclose quotes (ISOL) method requires two major accelerator components: a high power (100 kW) driver device to produce radionuclides in a production target/ion source complex, and a secondary beam accelerator to produce beams of radioactive ions up to energies on the order of 10 MeV per nucleon over a broad mass range. In reviewing the technological challenges of such a facility, several types of modem linear accelerators appear well suited. This paper reviews the properties of the linacs currently under construction and those proposed for future facilities for use either as the driver device or the radioactive beam post-accelerator. Other choices of accelerators, such as cyclotrons, for either the driver or secondary beam devices of a radioactive beam complex will also be compared. Issues to be addressed for the production accelerator include the choice of ion beam types to be used for cost-effective production of radionuclides. For the post-accelerator the choice of ion source technology is critical and dictates the charge-to-mass requirements at the injection stage

Radioactive beams produced by the ISOL method: development for laser ionization and for surface ionization; Faisceaux exotiques par methode ISOL: developpements pour l'ionisation par laser et l'ionisation de surface

Energy Technology Data Exchange (ETDEWEB)

Hosni, Faouzi

2004-10-01

The works were carried out in the framework of the research program PARRNe (production of radioactive neutron-rich nuclei). This program aims to determine optimal conditions to produce intense beams of neutron-rich isotopes. This thesis treats multiple technical aspects related to the production of separate radioactive isotopes in line (ISOL). It deals mainly with the development of the target-source unit which is the key element for projects such as SPIRAL-2 or EURISOL.The first part presents the various methods using fission as production mode and compares them: fission induced by thermal neutrons, induced by fast neutrons and photofission. The experiment carried out at CERN validated the interest of the photofission as a promising production mode of radioactive ions. That is why the institute of nuclear physics of Orsay decided to build a linear electron accelerator at the Tandem d'Orsay (ALTO).The second part of this thesis deals with the development of uranium targets. The X-rays diffraction and Scanning Electron Microscopy have been used as analysis techniques. They allowed to determine the chemical and structural characteristics of uranium carbide targets as function of various heating temperatures. After the production, the process of ionization has been studied. Two types of ion source have been worked out: the first one is a surface ion source and the second one is a source based on resonant ionization by laser. These two types of sources will be used for the ALTO project. (author)

Status of stable isotope enrichment, products, and services at the Oak Ridge National Laboratory

International Nuclear Information System (INIS)

Aaron, W.S.; Tracy, J.G.; Collins, E.D.

1997-01-01

The Oak Ridge national laboratory (ORNL) has been supplying enriched stable and radioactive isotopes to the research, medical, and industrial communities for over 50 y. Very significant changes have occurred in this effort over the past several years, and, while many of these changes have had a negative impact on the availability of enriched isotopes, more recent developments are actually improving the situation for both the users and the producers of enriched isotopes. ORNL is still a major producer and distributor of radioisotopes, but future isotope enrichment operations to be conducted at the isotope enrichment facility (IEF)fwill be limited to stable isotopes. Among the positive changes in the enriched stable isotope area are a well-functioning, long-term contract program, which offers stability and pricing advantages; the resumption of calutron operations; the adoption of prorated conversion charges, which greatly improves the pricing of isotopes to small users; ISO 9002 registration of the IEF's quality management system; and a much more customer-oriented business philosophy. Efforts are also being made to restore and improve upon the extensive chemical and physical form processing capablities that once existed in the enriched stable isotope program. Innovative ideas are being pursued in both technical and administrative areas to encourage the beneficial use of enriched stable isotopes and the development of related technologies. (orig.)

Status of stable isotope enrichment, products, and services at the Oak Ridge National Laboratory

Science.gov (United States)

Scott Aaron, W.; Tracy, Joe G.; Collins, Emory D.

1997-02-01

The Oak Ridge National Laboratory (ORNL) has been supplying enriched stable and radioactive isotopes to the research, medical, and industrial communities for over 50 y. Very significant changes have occurred in this effort over the past several years, and, while many of these changes have had a negative impact on the availability of enriched isotopes, more recent developments are actually improving the situation for both the users and the producers of enriched isotopes. ORNL is still a major producer and distributor of radioisotopes, but future isotope enrichment operations to be conducted at the Isotope Enrichment Facility (IEF) will be limited to stable isotopes. Among the positive changes in the enriched stable isotope area are a well-functioning, long-term contract program, which offers stability and pricing advantages; the resumption of calutron operations; the adoption of prorated conversion charges, which greatly improves the pricing of isotopes to small users; ISO 9002 registration of the IEF's quality management system; and a much more customer-oriented business philosophy. Efforts are also being made to restore and improve upon the extensive chemical and physical form processing capablities that once existed in the enriched stable isotope program. Innovative ideas are being pursued in both technical and administrative areas to encourage the beneficial use of enriched stable isotopes and the development of related technologies.

Status of stable isotope enrichment, products, and services at the Oak Ridge National Laboratory

International Nuclear Information System (INIS)

Aaron, W.S.; Tracy, J.G.; Collins, E.D.

1996-01-01

The Oak Ridge National Laboratory (ORNL) has been supplying enriched stable and radioactive isotopes to the research, medical, and industrial communities for over 50 years. Very significant changes have occurred in this effort over the past several years, and, while many of these changes have had a negative impact on the availability of enriched isotopes, more recent developments are actually improving the situation for both the users and the producers of enriched isotopes. ORNL is still a major producer and distributor of radioisotopes, but future isotope enrichment operations conducted at the Isotope Enrichment Facility (IEF) will be limited to stable isotopes. Among the positive changes in the enriched stable isotope area are a well-functioning, long-term contract program, which offers stability and pricing advantages; the resumption of calutron operations; the adoption of prorated conversion charges, which greatly improves the pricing of isotopes to small users; SIO 9002 registration of the IEF's quality management system; and a much more customer-oriented business philosophy. Efforts are also being made to restore and improve upon the extensive chemical and physical form processing capabilities that once existed in the enriched stable isotope program. Innovative ideas are being pursued in both technical and administrative areas to encourage the beneficial use of enriched stable isotopes and the development of related technologies

Semiconductor studies by radioactive probe atoms

International Nuclear Information System (INIS)

Wichert, Thomas

2003-01-01

There are a growing number of experimental techniques that have in common the usage of radioactive isotopes for the characterization of semiconductors. These techniques deliver atomistic information about identity, formation, lattice environment, and electronic structure, as well as dynamics of defects and defect complexes. The results obtained by different hyperfine techniques are discussed in context with the study of intrinsic and extrinsic defects, i.e. of vacancies or self-interstitials and dopant or impurity atoms, respectively. In addition, the employment of electrical and optical techniques in combination with radioactive isotopes is presented

Resonant ionization by laser beams: application to ions sources and to study the nuclear structure of radioactive tellurium isotopes; Ionisation resonante par faisceaux laser: application aux sources d'ions et a l'etude de la structure des noyaux radioactifs de tellure

Energy Technology Data Exchange (ETDEWEB)

Sifi, R

2007-07-15

The radioactive ion beams that are produced through current isotope separators are well separated according to the A mass but not according to the Z parameter. The resonant ionization through laser beams applied to ion sources allows the production of radioactive ion beam in a very selective and efficient way by eliminating the isobaric contamination. The first chapter is dedicated to the resonant ionization by laser beams, we describe the principle, the experimental setting, the lasers used, the ionization schemes and the domain of application. The second chapter deals with the application of resonant ionization to laser ion sources for the production of radioactive ion beams. We present experimental tests performed for getting copper ion beams. Resonant ionization through laser is also used in the spectroscopy experiments performed at the Isolde (isotope separation on-line device) installation in CERN where more than 20 elements are ionized very efficiently. The technique is based on a frequency scanning around the excitation transition of the atoms in order to probe the hyperfine structure. Laser spectroscopy allows the determination of the hyperfine structure as well as the isotopic shift of atoms. In the third chapter the method is applied to the spectroscopy of tellurium atoms. First, we define the 2 parameters on which the extraction is based: charge radius and nuclear moments, then we present several theoretical models that we have used to assess our experimental results. (A.C.)

A method of and apparatus for, monitoring the radioactivity of a plurality of samples incorporating lower energy beta-emitting isotopes

International Nuclear Information System (INIS)

Warner, G.T.; Potter, C.G.

1981-01-01

A method for monitoring the radioactivity of a number of samples incorporating low energy beta-emitting isotopes which allows the simultaneous precipitation of many samples with a minimum of sample handling, is described. The samples are placed on a support so that they are not overlapping, the support and sample are permeated with liquid or gel scintillant and the sample areas are scanned. (U.K.)

Iron isotope composition of particles produced by UV-femtosecond laser ablation of natural oxides, sulfides, and carbonates.

Science.gov (United States)

d'Abzac, Francois-Xavier; Beard, Brian L; Czaja, Andrew D; Konishi, Hiromi; Schauer, James J; Johnson, Clark M

2013-12-17

The need for femtosecond laser ablation (fs-LA) systems coupled to MC-ICP-MS to accurately perform in situ stable isotope analyses remains an open question, because of the lack of knowledge concerning ablation-related isotopic fractionation in this regime. We report the first iron isotope analysis of size-resolved, laser-induced particles of natural magnetite, siderite, pyrrhotite, and pyrite, collected through cascade impaction, followed by analysis by solution nebulization MC-ICP-MS, as well as imaging using electron microscopy. Iron mass distributions are independent of mineralogy, and particle morphology includes both spheres and agglomerates for all ablated phases. X-ray spectroscopy shows elemental fractionation in siderite (C-rich agglomerates) and pyrrhotite/pyrite (S-rich spheres). We find an increase in (56)Fe/(54)Fe ratios of +2‰, +1.2‰, and +0.8‰ with increasing particle size for magnetite, siderite, and pyrrhotite, respectively. Fe isotope differences in size-sorted aerosols from pyrite ablation are not analytically resolvable. Experimental data are discussed using models of particles generation by Hergenröder and elemental/isotopic fractionation by Richter. We interpret the isotopic fractionation to be related to the iron condensation time scale, dependent on its saturation in the gas phase, as a function of mineral composition. Despite the isotopic variations across aerosol size fractions, total aerosol composition, as calculated from mass balance, confirms that fs-LA produces a stoichiometric sampling in terms of isotopic composition. Specifically, both elemental and isotopic fractionation are produced by particle generation processes and not by femtosecond laser-matter interactions. These results provide critical insights into the analytical requirements for laser-ablation-based stable isotope measurements of high-precision and accuracy in geological samples, including the importance of quantitative aerosol transport to the ICP.

Stable isotope variations in benthic primary producers along the Bosphorus (Turkey): A preliminary study

International Nuclear Information System (INIS)

Calizza, Edoardo; Aktan, Yelda; Costantini, Maria Letizia; Rossi, Loreto

2015-01-01

Highlights: • Nitrogen pollution along the Bosphorus Strait was investigated. • C and N isotopic and elemental analyses on benthic primary producers were performed. • δ 15 N decreased, while δ 13 C and N% increased from north to south along the Strait. • Ulva lactuca was more useful than epiphytes as indicator of nitrogen pollution. • Preliminary isotopic analyses on resident organisms are useful monitoring tools. - Abstract: The Bosphorus Strait is a dynamic and complex system. Recent evidences showed nitrogen and heavy metal concentrations to follow opposite patterns across the Strait, suggesting a complex spatial organisation of the anthropogenic disturbance in this system. Here, we provide isotopic information on the origin and transportation of dissolved nitrogen along the Bosphorus. C and N isotopic and elemental analyses were performed on specimens of Ulva lactuca and associated epiphytes sampled in five locations across the Strait. Variations in C and N isotopic signatures were observed in U. lactuca, pointing to a decrease in the availability of anthropogenic organic dissolved nitrogen along a north-south direction. Conversely, epiphytes did not show isotopic or elemental patterns across the Strait. These results suggest that preliminary stable isotope surveys in extended costal systems basing on U. lactuca can represent a valuable tool to focus meaningful targets and hypotheses for pollution studies in the Mediterranean region

Experiments with SIRA - the radioactive ion separator

International Nuclear Information System (INIS)

Angelique, J.C.; Orr, N.A.

1998-01-01

There are two main techniques to obtain radioactive ion beams. One, consisting in the fragmentation of projectile in a thin target followed by a separation carried out with LISE or SISSI type spectrometers or by an alpha spectrometer is used currently at GANIL. The second one, the ISOL (Isotope Separator One-Line) is presently under study on the SIRa benchmark, as part of the SPIRaL (Source de Production d'Ions Radioactifs en Ligne). A high energy light ion beam is stopped by a thick target to produce radioactive nuclei by various reactions in the target. The target, usually of carbon, is heated at around 1800 deg. C in order to accelerate the migration of the atoms produced at the target surface. These atoms are then diffused by a transfer tube up to plasma region where they are ionized and then accelerated. As projectiles the GANIL project makes use of a large variety of heavy ions. A table containing the radioactive ion beam characteristics (charge state and lifetime), the primary beams, the yields and the expected intensities to be obtained with SPIRaL is presented. Also, data concerning the production rates of rare gases obtained during 1993 to 1994 are given

Overview of the U.S. Department of Energy's Isotope Programs

International Nuclear Information System (INIS)

Carty, J.

2004-01-01

This presentation provides an overview of the U.S. Department of Energy's Isotopes Program. The charter of the Isotope Programs covers the production and sale of radioactive and stable isotopes, associated byproducts, surplus materials, and related isotope services

Spes: An intense source of Neutron-Rich Radioactive Beams at Legnaro

Science.gov (United States)

Andrighetto, A.; Manzolaro, M.; Corradetti, S.; Scarpa, D.; Monetti, A.; Rossignoli, M.; Ballan, M.; Borgna, F.; D'Agostini, F.; Gramegna, F.; Prete, G.; Meneghetti, G.; Ferrari, M.; Zenoni, A.

2018-02-01

The Isotope Separation On-Line (ISOL) method for the production of Radioactive Ion Beams (RIB) is attracting significant interest in the worldwide nuclear physics community. Within this context the SPES (Selective Production of Exotic Species) RIB facility is now under construction at INFN LNL (Istituto Nazionale di Fisica Nucleare Laboratori Nazionali di Legnaro). This technique is established as one of the main techniques for high intensity and high quality beams production. The SPES facility will produce n-rich isotopes by means of a 40 MeV proton beam, emitted by a cyclotron, impinging on a uranium carbide multi-foil fission target. The aim of this work is to describe the most important results obtained by the study of the on-line behavior of the SPES production target assembly. This target system will produce RIBs at a rate of about 1013 fissions per second, it will be able to dissipate a total power of up to 10 kW, and it is planned to work continuously for 2 week-runs of irradiation. ISOL beams of 24 different elements will be produced, therefore a target and ion source development is ongoing to ensure a great variety of produced isotopes and to improve the beam intensity and purity.

Cluster decay of 218U isotope

International Nuclear Information System (INIS)

Shivakumaraswamy, G.; Umesh, T.K.

2012-01-01

The phenomenon of spontaneous emission of charged particles heavier than alpha particle and lighter than a fission fragment from radioactive nuclei without accompanied by the emission of neutrons is known as cluster radioactivity or exotic radioactivity. The process of emission of charged particles heavier than alpha particle and lighter than a fission fragment is called exotic decay or cluster decay. The phenomenon of cluster radioactivity was first predicted theoretically by Sandulescu et al in 1980. Rose and Jones made first experimental observations of 14 C emission from 223 Ra in 1984. Several cluster decay modes in trans-lead region have been experimentally observed. The half-life values for different modes of cluster decay from different isotopes of uranium have been calculated using different theoretical models such as the analytical super asymmetric model (ASAFM), Preformed cluster model (PCM) and Coulomb and Proximity potential model (CPPM) etc. Recently some semi-empirical formulae, i.e, single line of universal curve (UNIV), Universal decay law (UDL) for both alpha and cluster radioactivity have also been proposed to explain cluster decay data. The alpha decay half-life of 218-219 U isotopes has been experimentally measured in 2007. The half-life values for different cluster decay modes of 218 U isotopes have been calculated PCM model. Recently in 2011, the half-life values have also been calculated for some cluster decay modes of 222-236 U isotopes using the effective liquid drop description with the varying mass asymmetry (VMAS) shape and effective inertial coefficient. In the light of this, in the present work we have studied the cluster radioactivity of 218 U isotope. The logarithmic half-lives for few cluster decay modes from 218 U isotope have been calculated by using three different approaches, i.e, UNIV proposed by Poenaru et al in 2011, UDL proposed by Qi et al in 2009 and the CPPM model proposed by Santhosh et al in 2002. The CPPM based

Long-lived radioactive waste and nuclear plant decommissioning a legacy to future generations

International Nuclear Information System (INIS)

McAulay, I.R.

1996-01-01

Radioactive waste is an inevitable by-product of all uses of radioactive substances. This is the case of natural radioactivity as well as for artificially produced radioactive isotopes, and it is easy to overlook the significance of the waste problem in the case of technologically enhanced natural radioactivity. Several options are available for the disposal of radioactive waste and the paper considers these in detail from the point of view of the possible future impact of radiation doses to individuals or populations. Particular consideration is given to the use of deep disposal at stable geological sites as a means of dealing with large amounts of radioactive waste. It should not be forgotten that some of what we term waste today need not necessarily always be so. Indeed, there is a good case to make for the recycling of low activity materials rather than the uneconomic expedient of burying them. The paper will consider the possible recycling of valuable materials following suitable reprocessing and dilution and mention the dose implications of examples of such re-utilisation of radioactive materials

Long-lived radioactive waste and nuclear plant decommissioning a legacy to future generations

Energy Technology Data Exchange (ETDEWEB)

McAulay, I R [Trinity Coll., Dublin (Ireland). Physical Lab.

1996-10-01

Radioactive waste is an inevitable by-product of all uses of radioactive substances. This is the case of natural radioactivity as well as for artificially produced radioactive isotopes, and it is easy to overlook the significance of the waste problem in the case of technologically enhanced natural radioactivity. Several options are available for the disposal of radioactive waste and the paper considers these in detail from the point of view of the possible future impact of radiation doses to individuals or populations. Particular consideration is given to the use of deep disposal at stable geological sites as a means of dealing with large amounts of radioactive waste. It should not be forgotten that some of what we term waste today need not necessarily always be so. Indeed, there is a good case to make for the recycling of low activity materials rather than the uneconomic expedient of burying them. The paper will consider the possible recycling of valuable materials following suitable reprocessing and dilution and mention the dose implications of examples of such re-utilisation of radioactive materials.

METHOD FOR PRODUCING ISOTOPIC METHANES AND PARTIALLY HALOGENATED DERIVATIVES THEROF

Science.gov (United States)

Frazer, J.W.

1959-08-18

A method is given for producing isotopic methanes and/ or partially halogenated derivatives. Lithium hydride, deuteride, or tritide is reacted with a halogenated methane or with a halogenated methane in combination with free halogen. The process is conveniently carried out by passing a halogenated methane preferably at low pressures or in an admixture with an inert gas through a fixed bed of finely divided lithium hydride heated initially to temperatures of 100 to 200 deg C depending upon the halogenated methane used.

Osmium isotopic tracing of atmospheric emissions from an aluminum smelter

Science.gov (United States)

Gogot, Julien; Poirier, André; Boullemant, Amiel

2015-09-01

We present for the first time the use of osmium isotopic composition as a tracer of atmospheric emissions from an aluminum smelter, where alumina (extracted from bauxite) is reduced through electrolysis into metallic aluminum using carbonaceous anodes. These anodes are consumed in the process; they are made of petroleum coke and pitch and have high Re/Os elementary ratio. Due to the relatively large geological age of their source material, their osmium shows a high content of radiogenic 187Os produced from in situ187Re radioactive decay. The radiogenic isotopic composition (187Os/188Os ∼ 2.5) of atmospheric particulate emissions from this smelter is different from that of other typical anthropogenic osmium sources (that come from ultramafic geological contexts with unradiogenic Os isotopes, e.g., 187Os/188Os < 0.2) and also different from average eroding continental crust 187Os/188Os ratios (ca. 1.2). This study demonstrates the capacity of osmium measurements to monitor particulate matter emissions from the Al-producing industry.

Benchmark studies of induced radioactivity and remanent dose rates produced in LHC materials

International Nuclear Information System (INIS)

Brugger, M.; Mayer, S.; Roesler, S.; Ulrici, L.; Khater, H.; Prinz, A.; Vincke, H.

2005-01-01

Samples of materials that will be used for elements of the LHC machine as well as for shielding and construction components were irradiated in the stray radiation field of the CERN-EU high-energy Reference Field facility. The materials included various types of steel, copper, titanium, concrete and marble as well as light materials such as carbon composites and boron nitride. Emphasis was put on an accurate recording of the irradiation conditions, such as irradiation profile and intensity, and on a detailed determination of the elemental composition of the samples. After the irradiation, the specific activity induced in the samples as well as the remanent dose rate were measured at different cooling times ranging from about 20 minutes to two months. Furthermore, the irradiation experiment was simulated using the FLUKA Monte Carlo code and specific activities. In addition, dose rates were calculated. The latter was based on a new method simulating the production of various isotopes and the electromagnetic cascade induced by radioactive decay at a certain cooling time. In general, solid agreement was found, which engenders confidence in the predictive power of the applied codes and tools for the estimation of the radioactive nuclide inventory of the LHC machine as well as the calculation of remanent doses to personnel during interventions. (authors)

Moessbauer Effect applications using intense radioactive ion beams

International Nuclear Information System (INIS)

Taylor, R.D.

1990-01-01

The Moessbauer Effect is reviewed as a promising tool for a number of new solid state studies when used in combination with radioactive beam/implantation facilities. The usual Moessbauer Effect involves long-lived radioactive parents (days to years) that populate low-lying nuclear excited states that subsequently decay to the ground state. Resonant emission/absorption of recoil-free gamma rays from these states provide information on a number of properties of the host materials. Radioactive ion beams (RIB) produced on-line allow new Moessbauer nuclei to be studied where there is no suitable parent. The technique allows useful sources to be made having extremely low local concentrations. The ability to separate the beams in both Z and A should provide high specific activity ''conventional'' sources, a feature important in some applications such as Moessbauer studies in diamond anvil high pressure cells. Exotic chemistry is proposed using RIB and certain Krypton and Xenon Moessbauer isotopes

Radioactivity in the environment

International Nuclear Information System (INIS)

Costello, J.M.

1983-01-01

Radioactivity is a natural phenomenon. Out of 1700 known isotopes of 104 chemical elements, only about 16 per cent are stable. Seventy-three radioactive isotopes of 39 elements occur naturally in the terrestrial environment. The significance of environmental radioactivity lies in the contribution to the annual exposure of the general population to ionising radiation. This exposure results largely from natural sources of radioactivity and radiation together with applications of radiation in medicine. Minor contributions are from nuclear weapons tests, nuclear power production and the nuclear fuel cycle, and consumer products including luminous clocks and watches, television receivers and smoke detectors. The natural background radiation level varies substantially with altitude and geographic location. Although no satisfactory evidence is available that natural variations in background radiation levels are detrimental to humans, upper limits of risk have been estimated for possible somatic and genetic effects from these levels of radiation. Contributory sources of and variability in the radiation background are reviewed and the relation between effective dose equivalent and associated detriment outlined. The risk from exposure to an average level of background radiation is compared with risks from other human activities

Source of radioactivity in the ocean environment

International Nuclear Information System (INIS)

Solomon, K.A.

1988-01-01

This paper summarizes both natural and man-made radioactivity in the marine environment. Radioactivity occurs naturally in both the sea water and in the ocean sediment. Radioactivity in the sea water is fairly uniform geographically and is dominated by the naturally occurring isotope 40/K (potassium-40). Unlike sea water, sediment radiation levels vary with sediment type and location. The primary source of natural radiation in the sediment results from deposition of insoluble thorium isotopes formed by the decay of water-soluble uranium. Man-made sources of radioactivity arise from, in descending order of importance: - sinking of two U.S. and two Soviet nuclear submarines; fallout from nuclear weapons testing; dumping of primarily British and Americal low-level nuclear waste; and dumping of reprocessing plant radiated effluents from the British Windscale facility and other European and Indian reprocessing facilities. 1 table

Radioactive 85Kr in krypton enriched with a light isotope

International Nuclear Information System (INIS)

Kuz'minov, V.V.; Novikov, V.M.; Pomanskii, A.A.; Pritychenko, B.V.; Vieiar, J.; Garcia, E.; Morales, A.; Morales, J.; Nunes-Lagos, R.; Piumendon, J.

1993-01-01

Radioactive krypton 85, a product of nuclear power generation, is known to be accumulating in the atmosphere continuously. Its volumetric activity in natural krypton is 700-800 Bq/liter. This can cause difficulties, e.g., in the fabrication of nuclear radiation detector for high-mass krypton. Krypton with a reduced 85 Kr content can be obtained by isotope separation. As part of an experiment to look for two-positron decay and conversion of an atomic electron to a positron in 78 Kr, Saenz measured the 85 Kr content in 78 Kr-enriched krypton. A mixture of two 85 Kr samples was used as the working substance of a cylindrical ionization chamber. The useful volume (1.33 liter) of the chamber contained 35.3 liters of gas at ∼2.5 kPa. The energy resolution of the detector at an energy of 0.511 MeV was 3.8%. The measurements were made in a passive lead shield 20 cm thick in an underground laboratory at a depth of 675 m water equivalent. Results are presented for counting rates in low-energy regions, contribution of krypton-85 to background, and the volumetric activity of krypton-85

Physics and Technology for the Next Generation of Radioactive Ion Beam Facilities: EURISOL

CERN Document Server

Kadi, Y; Catherall, R; Giles, T; Stora, T; Wenander, F K

2012-01-01

Since the discovery of artificial radioactivity in 1935, nuclear scientists have developed tools to study nuclei far from stability. A major breakthrough came in the eighties when the first high energy radioactive beams were produced at Berkeley, leading to the discovery of neutron halos. The field of nuclear structure received a new impetus, and the major accelerator facilities worldwide rivalled in ingenuity to produce more intense, purer and higher resolution rare isotope beams, leading to our much improved knowledge and understanding of the general evolution of nuclear properties throughout the nuclear chart. However, today, further progress is hampered by the weak beam intensities of current installations which correlate with the difficulty to reach the confines of nuclear binding where new phenomena are predicted, and where the r-process path for nuclear synthesis is expected to be located. The advancement of Radioactive Ion Beam (RIB) science calls for the development of so-called next-generation facil...

Use of stable and radioactive isotopes in the determination of the recharge rate in Djeffara aquifer system southern Tunisia

International Nuclear Information System (INIS)

Trabelisi, R.; Zouari, K.

2012-12-01

Southern Tunisia is characterized by the presence of several hydrogeological basins, which extend over Tunisian borders. The Djeffara aquifer is one of the most important aquifer systems n this area and contains several interconnected aquifer levels. Stable (δ 2 H, δ 18 O and δ 13 C) and radioactive isotopes (1 4C , 3 H ) have been used to evaluate recharge mechanisms and groundwater residence time in the Djeffara multi-aquifer. Thesis aquifer presents two compartments, the first one ( west of the Medenine fault system) is unconfined with a well defined isotope fingerprint, the second compartment is deeper and confined multi- tracer results show groundwater of different origins, and ages , and that tectonic features control ground water flows. The unconfined part was mostly recharged during the Holocene. The recharge rates of this aquifer, inferred by 1 4C ages, are variable and could reach 3.5 mm/year. However, stable isotope composition and 1 4 'C content of the confined groundwater indicates carrier recharge during late pelistocene cold periods. (Author)

Development and test of a cryogenic trap system dedicated to confinement of radioactive volatile isotopes in SPIRAL2 post-accelerator

Science.gov (United States)

Souli, M.; Dolégiéviez, P.; Fadil, M.; Gallardo, P.; Levallois, R.; Munoz, H.; Ozille, M.; Rouillé, G.; Galet, F.

2011-12-01

A cryogenic trap system called Cryotrap has been studied and developed in the framework of nuclear safety studies for SPIRAL2 accelerator. The main objective of Cryotrap is to confine and reduce strongly the migration of radioactive volatile isotopes in beam lines. These radioactive gases are produced after interaction between a deuteron beam and a fissile target. Mainly, Cryotrap is composed by a vacuum vessel and two copper thermal screens maintained separately at two temperatures T1=80 K and T2=20 K. A Cryocooler with two stages at previous temperatures is used to remove static heat losses of the cryostat and ensure an efficient cooling of the system. Due to strong radiological constraints that surround Cryotrap, the coupling system between Cryocooler and thermal screens is based on aluminum thermo-mechanical contraction. The main objective of this original design is to limit direct human maintenance interventions and provide maximum automated operations. A preliminary prototype of Cryotrap has been developed and tested at GANIL laboratory to validate its design, and determine its thermal performance and trapping efficiency. In this paper, we will first introduce briefly SPIRAL2 project and discuss the main role of Cryotrap in nuclear safety of the accelerator. Then, we will describe the proposed conceptual design of Cryotrap and its main characteristics. After that, we will focus on test experiment and analyze experimental data. Finally, we will present preliminary results of gas trapping efficiency tests.

Radioactive ion beams produced by neutron-induced fission at ISOLDE

CERN Document Server

Catherall, R; Gilardoni, S S; Köster, U

2003-01-01

The production rates of neutron-rich fission products for the next-generation radioactive beam facility EURISOL are mainly limited by the maximum amount of power deposited by protons in the target. An alternative approach is to use neutron beams to induce fission in actinide targets. This has the advantage of reducing: the energy deposited by the proton beam in the target; contamination from neutron-deficient isobars that would be produced by spallation; and mechanical stress on the target. At ISOLDE CERN, tests have been made on standard ISOLDE actinide targets using fast neutron bunches produced by bombarding thick, high-Z metal converters with 1 and 1.4 GeV proton pulses. This paper reviews the first applications of converters used at ISOLDE. It highlights the different geometries and the techniques used to compare fission yields produced by the proton beam directly on the target with neutron-induced fission. Results from the six targets already tested, namely UC2/graphite and ThO2 targets with tungsten an...

Isotope hydrology of catchment basins: lithogenic and cosmogenic isotopic systems

Energy Technology Data Exchange (ETDEWEB)

Nimz, G. J., LLNL

1998-06-01

A variety of physical processes affect solute concentrations within catchment waters. The isotopic compositions of the solutes can indicate which processes have determined the observed concentrations. These processes together constitute the physical history of the water. Many solutes in natural waters are derived from the interaction between the water and the rock and/or soil within the system - these are termed `lithogenic` solutes. The isotopic compositions of these solutes provide information regarding rock-water interactions. Many other solutes have their isotopic compositions determined both within and outside of the catchment - i.e., in addition to being derived from catchment rock and soil, they are solutes that are also transported into the catchment. Important members of this group include solutes that have isotopic compositions produced by atomic particle interactions with other nuclides. The source of the atomic particles can be cosmic radiation (producing `cosmogenic` nuclides in the atmosphere and land surface), anthropogenic nuclear reactions (producing `thermonuclear` nuclides), or radioactive and fission decay of naturally-occurring elements, principally {sup 238}U (producing `in-situ` lithogenic nuclides in the deep subsurface). Current language usage often combines all of the atomic particle-produced nuclides under the heading `cosmogenic nuclides`, and for simplicity we will often follow that usage here, although always indicating which variety is being discussed. This paper addresses the processes that affect the lithogenic and cosmogenic solute concentrations in catchment waters, and how the isotopic compositions of the solutes can be used in integrative ways to identify these processes, thereby revealing the physical history of the water within a catchment system. The concept of a `system` is important in catchment hydrology. A catchment is the smallest landscape unit that can both participate in all of the aspects of the hydrologic cycle and

The future of the accelerator mass spectrometry of rare long-lived radioactive isotopes

International Nuclear Information System (INIS)

Litherland, A.E.

1990-01-01

Accelerators, originally designed for nuclear physics, can be added to mass spectrometric apparatus to increase the sensitivity so that isotope ratios in the range 10 -12 to 10 -15 can be measured routinely. This significant improvement of high-sensitivity mass spectrometry has been called Accelerator Mass Spectrometry. The present article addresses the basic principles of accelerator mass spectrometry and some recent applications which show its versatility. In particular, it is noted that accelerator mass spectrometry could play an increasing role in the measurement of the levels of long lived radioactivities in the environment, including the actinides, which result from human activities such as the use of nuclear power. To fulfill this promise, continued research and development is necessary to provide ion sources, various types of heavy ion accelerators and peripheral magnetic and electric analysers. (N.K.)

A radioactive ion beam facility using photofission

CERN Document Server

Diamond, W T

1999-01-01

Use of a high-power electron linac as the driver accelerator for a Radioactive Ion Beam (RIB) facility is proposed. An electron beam of 30 MeV and 100 kW can produce nearly 5x10 sup 1 sup 3 fissions/s from an optimized sup 2 sup 3 sup 5 U target and about 60% of this from a natural uranium target. An electron beam can be readily transmitted through a thin window at the exit of the accelerator vacuum system and transported a short distance through air to a water-cooled Bremsstrahlung-production target. The Bremsstrahlung radiation can, in turn, be transported through air to the isotope-production target. This separates the accelerator vacuum system, the Bremsstrahlung target and the isotope-production target, reducing remote handling problems. The electron beam can be scanned over a large target area to reduce the power density on both the Bremsstrahlung and isotope-production targets. These features address one of the most pressing technological challenges of a high-power RIB facility, namely the production o...

Radioactive ion beams and techniques for solid state research

International Nuclear Information System (INIS)

Correia, J.G.

1998-01-01

In this paper we review the most recent and new applications of solid state characterization techniques using radioactive ion beams. For such type ofresearch, high yields of chemically clean ion beams of radioactive isotopesare needed which are provided by the on-line coupling of high resolution isotope separators to particle accelerators, such as the isotope separator on-line (ISOLDE) facility at CERN. These new experiments are performed by an increasing number of solid state groups. They combine nuclear spectroscopic techniques such as Moessbauer, perturbed angular correlations (PAC) and emission channeling with the traditional non-radioactive techniques liked deep level transient spectroscopy (DLTS) and Hall effect measurements. Recently isotopes of elements, not available before, were successfully used in new PAC experiments, and the first photoluminescence (PL) measurements, where the element transmutation plays the essential role on the PL peak identification, have been performed. The scope of applications of radioactive ion beams for research in solid state physics will be enlarged in the near future, with the installation at ISOLDE of a post-accelerator device providing radioactive beams with energies ranging from a few keV up to a few MeV. (orig.)

Development of isotope hydrology technology in China

International Nuclear Information System (INIS)

Li Zhangsu

1988-01-01

The development of isotope hydrology technology in China is described. The isotope technology provides an independent approach for solving hydrological problems. Isotope hydrology is applied in three ways: the use of change in environmental isotopic composition of water (especially used in water resources exploitation), the use of artificial radioactive tracers and the use of redioisotope instruments. Many important achievements have been obtained in application of isotopic hydrology technology. For the sake of promoting rapid development of isotope hydrology the topics on management, technology and others are commented

Use of Eichornia crassipes for treatment of low level liquid radioactive waste

Energy Technology Data Exchange (ETDEWEB)

Hafez, N.; Ramadan, Y.S.; Hassanin, R.A.; Gafez, M.B. (Atomic Energy Authority, Hot Lab. Center, Cairo (Egypt))

1993-01-01

Radioactive and non-radioactive isotopes of cobalt, cerium and cesium were found to be accumulated inside Eichornia crassipes (the water hyacinth). The rate and extent of accumulation were dependent upon environmental parameters such as pH, temperature and interference by certain anions and cations. The accumulation rate of radioactive isotopes inside Eichornia crassipes, were more rapid than non-active ions. The results showed that accumulation of such metals inside the plant could be used successfully in the treatment of low-level liquid radioactive wastes. (author) 4 figs., 2 tabs., 15 refs.

Use of Eichornia crassipes for treatment of low level liquid radioactive waste

International Nuclear Information System (INIS)

Hafez, N.; Ramadan, Y.S.; Hassanin, R.A.; Gafez, M.B.

1993-01-01

Radioactive and non-radioactive isotopes of cobalt, cerium and cesium were found to be accumulated inside Eichornia crassipes (the water hyacinth). The rate and extent of accumulation were dependent upon environmental parameters such as pH, temperature and interference by certain anions and cations. The accumulation rate of radioactive isotopes inside Eichornia crassipes, were more rapid than non-active ions. The results showed that accumulation of such metals inside the plant could be used successfully in the treatment of low-level liquid radioactive wastes. (author) 4 figs., 2 tabs., 15 refs

Radioactive isotopes in occupational health

International Nuclear Information System (INIS)

Favino, Angelo.

1976-01-01

It is highly desirable today to know and use for industrial medicine purposes all scientific and technological data available in the field of nuclear medicine. The present textbook is an inventory of all possibilities given to occupational doctors in order to pronounce a judgement of ability to work on the occasion of preemployment or routine medical examinations. Such applications require a high degree of competence in radiological protection and also require observation of the basic Safety Standards of Euratom and of the recommendations of the International Committee on Radiological Protection, the same safety principles having been incorporated in all the legislations of the Member States of the Community. In this book a number of chapters are devoted to the description of the basic principles for maximum permissible doses, dosimetric surveillance, medical supervision of workers exposed to ionizing radiations, and medical treatments to be used after a radioactive contamination. In addition a small number of preventive measures are described for all utilisations of radioactive substances for diagnostic or therapeutic purposes

Is Radioactive Decay Really Exponential?

OpenAIRE

Aston, Philip J.

2012-01-01

Radioactive decay of an unstable isotope is widely believed to be exponential. This view is supported by experiments on rapidly decaying isotopes but is more difficult to verify for slowly decaying isotopes. The decay of 14C can be calibrated over a period of 12,550 years by comparing radiocarbon dates with dates obtained from dendrochronology. It is well known that this approach shows that radiocarbon dates of over 3,000 years are in error, which is generally attributed to past variation in ...

Production of krypton isotopes by (p,xn) reactions on bromine

International Nuclear Information System (INIS)

Chiengmai, S.N.; Hans, L.; Petter, M.

1976-06-01

Radioactive isotopes of the halogens are of great importance when preparing radiopharmaceuticals. 77 Br has mainly been produced by a direct reaction 75 As(α,2n) 77 Br. Recently an indirect way, producing 77 Kr which then decays to 77 Br, has been suggested. Since this provides a convenient method of separation this work develops this idea further making use of high energy protons on bromine Br(p,xn) 77 Kr→ 77 Br. The production cross-section for this reaction has been studied in the proton-energy interval of 20-80 MeV and the optimal production procedures considered. (Auth.)

Technical testing of portable isotope identification instruments

International Nuclear Information System (INIS)

Smith, D.E.

2001-01-01

Full text: The United States Customs Service has, as a part of its mission, the protection of the borders of the United States from the import or export of illicit radioactive materials. Of paramount importance is the ability to interdict the smuggling of special nuclear material, nuclear weapons and other radioactive materials that could be used as a weapon of mass destruction against the population and infrastructure of the U.S. or another country. Radiation detection technology exists in the form of pocket size, hand-held and portal radiation detectors that have the ability to detect radiation with great sensitivity and low false alarm rates. U.S. Customs has chosen to implement pocket size detectors or radiation pagers as the personal tool of each inspector for the detection of radioactive material. In the search for illicit shipment of radioactive materials, innocent radiation detections may occur with some frequency due to common radioactive sources that may be encountered in day to day living. Examples include lantern mantles, some camera lenses, welding rods, certain dishware containing uranium glaze, and natural marble objects such as statues or architectural pieces. Perhaps the most common innocent detection encountered at the border and in public areas in general is due to the in vivo placement of radioactive sources for use in nuclear medicine therapy and diagnostics. Outpatients from such therapy can remain detectable for three weeks or more. Also, legal shipments of radioisotopes are common occurrences in cargo and express mail shipments. The customs inspector who detects radioactive material in the course of his duties must decide whether detection is innocent; is indicative of a nuclear device or special nuclear material; or whether the source could be injurious to him/her or the general public. It is at this point that a portable instrument capable of identifying gamma or neutron emitting isotopes is essential to the customs examination procedure

Mass measurement of radioactive isotopes

CERN Document Server

Kluge, H J; Scheidenberger, C

2004-01-01

The highest precision in mass measurements on short-lived radionuclides is obtained using trapping and cooling techniques. Here, the experimental storage ring (ESR) at GSI/Darmstadt and the tandem Penning trap mass spectrometer ISOLTRAP at ISOLDE/CERN play an important role. Status and recent results on mass measurements of radioactive nuclides with ESR and ISOLTRAP are summarized.

State of radionuclides in seawater. Comparison of natural stable and artificial radioactive isotope s of mercury and zinc in natural waters of the arid zone of the USSR

International Nuclear Information System (INIS)

Rakhmatov, U; Khikmatov, K; Kist, A.A.; Kulmatov, R.A.; Teshabaev, S.T.; Volkov, A.A.

1986-01-01

This paper studies the state of stable and artificial radioactive isotopes of merury and zinc in natural waters of the arid zone of the USSR by radioactivity and radiochemical methods. Convergent results have been obtained for the dissolved forms of mercury and zinc in natural waters of the arid zone in a comparison of the results of radioactivation analysis and laboratory simulation using the radionuclides mercury-203 and zinc-65

Secondary ion mass spectrometry and environment. SIMS as applied to the detection of stable and radioactive isotopes in marine organisms

International Nuclear Information System (INIS)

Chassard-Bouchaud, C.; Escaig, F.; Hallegot, P.

1984-01-01

Several marine species of economical interest, Crustacea (crabs and prawns) and Molluscs (common mussels and oysters) were collected from coastal waters of France: English Channel, Atlantic Ocean and Mediterranean Sea and of Japan. Microanalyses which were performed at the tissue and cell levels, using Secondary Ion Mass Spectrometry, revealed many contaminants; stable isotopes as well as radioactive actinids such as uranium were detected. Uptake, storage and excretion target organs were identified [fr

Isotope ratios as pollutant source and behaviour indicators

International Nuclear Information System (INIS)

1975-01-01

Recent years have witnessed significant advances in isotope techniques for identifying origins and for studying the behaviour of trace contaminants and pollutants of the environment under actual existing environmental conditions. Improvements in the supply of stable isotopes and their labelled compounds, instrumental analysis and information on stable or radioactive isotopic ratios of existing environmental contaminants as a function of origin or behaviour have provided relatively new tools for the environmental scientist. While variations in natural or existing environmental stable and radioactive nuclides could be regarded as 'background noise' in conventional tracer experiments they promised unique information about sources and behaviour to those who listened carefully. (author)

A target concept for intense radioactive beams in the 132Sn Region

International Nuclear Information System (INIS)

Nolen, J.A. Jr.

1993-01-01

To produce intense secondary beams of radioactive isotopes, primary beams of up to 100 kW are being proposed at some facilities. There are plans to test production targets with 800 MeV protons at such higher power at the Rutherford Appleton Laboratory. In this paper the use of high energy neutrons as a possible alternative is presented. The concept is to generate an intense beam of neutrons in a well-cooled target with a primary deuteron beam. The neutrons have a high cross section for producing fission fragments in a thick uranium target which is coupled to the ion source for the secondary beams. The effective target thickness is large and the power dissipated in the ISOL target is relatively small, which should lead to intense beams of neutron-rich, intermediate-mass isotopes such as 132 Sn

Manual to radioactive waste management produced in hospitals, research and education centers

International Nuclear Information System (INIS)

Villasenor N, L.F.; Mejia L, M.

1996-01-01

This manual collects the experience on the disposal and management of the wastes produced in the preparation and application of radioactive material. Although the content is not so extensive, the authors have tried to provide the necessary guidelines and adequate information for the management of the wastes produced in hospitals and research and education centers. The objective of this work is to describe the basis and principles for the establishment of a minimization program, a segregation program and a provisional waste storage, in order to reduce the generation of wastes, personal exposure and the environmental impact. (authors). 5 refs

FREEZE-OUT YIELDS OF RADIOACTIVITIES IN CORE-COLLAPSE SUPERNOVAE

International Nuclear Information System (INIS)

Magkotsios, Georgios; Wiescher, Michael; Timmes, F. X.

2011-01-01

We explore the nucleosynthesis trends from two mechanisms during freeze-out expansions in core-collapse supernovae. The first mechanism is related to the convection and instabilities within homogeneous stellar progenitor matter that is accreted through the supernova shock. The second mechanism is related to the impact of the supersonic wind termination shock (reverse shock) within the tumultuous inner regions of the ejecta above the proto-neutron star. Our results suggest that isotopes in the mass range 12 ≤ A ≤ 122 that are produced during the freeze-out expansions may be classified in two families. The isotopes of the first family manifest a common mass fraction evolutionary profile, whose specific shape per isotope depends on the characteristic transition between two equilibrium states (equilibrium state transition) during each type of freeze-out expansion. The first family includes the majority of isotopes in this mass range. The second family is limited to magic nuclei and isotopes in their locality, which do not sustain any transition, become nuclear flow hubs, and dominate the final composition. We use exponential and power-law adiabatic profiles to identify dynamic large-scale and small-scale equilibrium patterns among nuclear reactions. A reaction rate sensitivity study identifies those reactions that are crucial to the synthesis of radioactivities in the mass range of interest. In addition, we introduce non-monotonic parameterized profiles to probe the impact of the reverse shock and multi-dimensional explosion asymmetries on nucleosynthesis. Cases are shown in which the non-monotonic profiles favor the production of radioactivities. Non-monotonic freeze-out profiles involve longer non-equilibrium nucleosynthesis intervals compared with the exponential and power-law profiles, resulting in mass fraction trends and yield distributions that may not be achieved by the monotonic freeze-out profiles.

National Centre for Radioactive Ion Beams (NCRIB)

International Nuclear Information System (INIS)

Chintalapudi, S.N.

1999-01-01

A dedicated National Centre for RIB (NCRIB) proposed discussed at several forums is presented. The production of (RIB) radioactive ion beams and applications of beams leading to competitive studies in nuclear structure, nuclear reactions, condensed matter, bio-science and radioactive isotope production etc. are mentioned

Radioactive waste management and their ultimate disposal technologies in India: recent practices and developments

International Nuclear Information System (INIS)

Bajpai, R.K.

2015-01-01

The radioactive wastes that arise from the use of uranium, thorium and other radioactive isotopes during their various applications in the field of power generation, industry, agriculture and medicine are among the most talked about and at time even highly dreaded substances created by man in recent past. Most of the fears owe their genesis to extraordinary periods of time over which such waste remain radioactive and continue to emit radiations which are invisible to human eyes. These time periods run into tens of thousands of years and as a result any solution for management and permanent isolation of such waste needs to demonstrate safety of mankind and environment over such lengthy time frames. For example a radioactive isotope of strontium, known as 90 Sr takes about 300 years to loose its entire radioactivity. Similarly a popular isotope of plutonium 239 Pu needs almost 2.5 lakhs years to shed its entire radioactivity by converting itself to a non radioactive element. In this talk some salient aspects of radioactive waste management and solutions for their permanent isolation under consideration in India are discussed

Evaluation of management of radioactive waste in nuclear medicine department of radiation and isotopes center, Khartoum

International Nuclear Information System (INIS)

Ahmed, Amel Bushra Abaker

2001-01-01

Evaluation of management of radioactive waste in nuclear medicine department of radiation and isotopes center in Khartoum, Sudan, was conducted using radiation survey meter. The purpose of this study is to provide protection of workers, patients, co patients, an the environment by introducing good practice in management of radioactive waste generated in this lab. In this work measurement of radiation effective dose at different locations in the department were carried out. These locations were selected around the radioactive liquid and solid waste disposal position. It was found that the effective doses per year from radioactive wastes obtained through this work using the survey meter RDS-120 at these locations, are 1.47 mSv/y at the neighbouring patients room, 5.47 mSv/y at the hot lab., 0.09 mSv/y at the neighbouring toilet, 0.321 mSv/y at the water closet, and 1.4 mSv/y at the place down water closet. The results obtained shows that the dose levels waste at the location not exceed the recommended dose limits for workers 20 mSv/y, that set by basic safety standards (Bss 115) which published by the international atomic energy agency. Also it s comply with the national regulation, regulation on basic radiation protection requirement and dose limits 1996, issued by sudan atomic energy commission act 1996. The annual dose calculated for the patients and co-patients at rooms around the nuclear medicine department, the results shows that dose are fairly high. Measure should taken to improve the waste management in the department for better protection of workers, patients and co patients. (Author)

Detection systems for radioactive ion beams

International Nuclear Information System (INIS)

Savajols, H.

2002-01-01

Two main methods are used to produce radioactive ion beams: -) the ISOL method (isotope separation on-line) in which the stable beam interacts with a thick target, the reaction products diffuse outside the target and are transferred to a source where they are ionized, a mass separator and a post-accelerator drive the selected radioactive ions to the right energy; -) the in-flight fragmentation method in which the stable beam interacts with a thin target, the reaction products are emitted from the target with a restricted angular distribution and a velocity close to that of the incident beam, the experimenter has to take advantage from the reaction kinetics to get the right particle beam. Characteristic time is far longer with the ISOL method but the beam intensity is much better because of the use of a post-accelerator. In both cases, the beam intensity is lower by several orders of magnitude than in the case of a stable beam. This article presents all the constraints imposed by radioactive beams to the detection systems of the reaction products and gives new technical solutions according to the type of nuclear reaction studied. (A.C.)

Neutron spectra produced by moderating an isotopic neutron source

International Nuclear Information System (INIS)

Carrillo Nunnez, Aureliano; Vega Carrillo, Hector Rene

2001-01-01

A Monte Carlo study has been carried out to determine the neutron spectra produced by an isotopic neutron source inserted in moderating media. Most devices used for radiation protection have a response strongly dependent on neutron energy. ISO recommends several neutron sources and monoenergetic neutron radiations, but actual working situations have broad spectral neutron distributions extending from thermal to MeV energies, for instance, near nuclear power plants, medical applications accelerators and cosmic neutrons. To improve the evaluation of the dosimetric quantities, is recommended to calibrate the radiation protection devices in neutron spectra which are nearly like those met in practice. In order to complete the range of neutron calibrating sources, it seems useful to develop several wide spectral distributions representative of typical spectra down to thermal energies. The aim of this investigation was to use an isotopic neutron source in different moderating media to reproduce some of the neutron fields found in practice. MCNP code has been used during calculations, in these a 239PuBe neutron source was inserted in H2O, D2O and polyethylene moderators. Moderators were modeled as spheres and cylinders of different sizes. In the case of cylindrical geometry the anisotropy of resulting neutron spectra was calculated from 0 to 2 . From neutron spectra dosimetric features were calculated. MCNP calculations were validated by measuring the neutron spectra of a 239PuBe neutron source inserted in a H2O cylindrical moderator. The measurements were carried out with a multisphere neutron spectrometer with a 6LiI(Eu) scintillator. From the measurements the neutron spectrum was unfolded using the BUNKIUT code and the UTA4 response matrix. Some of the moderators with the source produce a neutron spectrum close to spectra found in actual applications, then can be used during the calibration of radiation protection devices

Availability of enriched stable isotopes: present status and future prospects

International Nuclear Information System (INIS)

Hoff, R.W.

1986-01-01

The Electromagnetic Isotope Enrichment Facility (EMIEF) is currently used to produce 225 enriched stable isotopes of 50 elements. Among these are included most of the known elements with stable isotopes except for the noble gases, certain light elements, monisotopic elements, etc. The EMIEF can also be used to produce enriched samples of radioactive species, most notably the isotopes of uranium and plutonium. These enriched materials are placed in either the Sales Inventory of in the Research Materials Collection (RMC). The materials in the Sales Inventory are for sale to anyone on a first come, first served basis. Prices in the most recent catalog range from $0.05/mg for 99.8% 140 Ce to $1,267/mg for 98.5% 176 Lu. The materials in the RMC are made available to US researchers (or groups that include a US investigator) on a loan basis for use in non-destructive experiments and applications. In addition, certain samples have been provided to European investigators for cross-section studies through the auspices of EURATOM and the European-American Nuclear Data Committee. The status of the enriched isotopes included in the Sales Inventory is tabulated where isotopes are listed that are either not available or are in insufficient quantity or quality to meet current requests, as of 6/30/86. These can be summarized in the following subcategories: isotopes with zero inventory (22), Isotopes of insufficient quantity (17), and isotopes with insufficient enrichment quality (10). Of these 49 species, the supplies of 10 will be replenished by the scheduled FY86 enrichments in process (isotopes of bromine, calcium, nickel, potassium, rubidium, and strontium). In Table 3 are listed isotopes where the current inventory is less than the average annual sales level for the past five years. There are 47 isotopes listed, representing 25 different elements. Thus, there exists considerable potential for a substantial increase in the number of isotopes with zero inventory

Total cross section measurement of radioactive isotopes with a thin beam neutron spectrometer

International Nuclear Information System (INIS)

Razbudej, V.F.; Vertebnyj, V.P.; Padun, G.S.; Muravitskij, A.V.

1975-01-01

The method for measuring the neutron total cross sections of radioactive isotopes by a time-of-flight spectrometer with a narrow (0.17 mm in diameter) beam of thermal neutrons is described. The distinguishing feature of this method is the use of capillary samples with a small amount of substance (0.05-1.0 mg). The energy range is 0.01-0.3 eV. The total cross sections of irradiated samples of sub(153)Eu and sub(151)Eu are measured. From them are obtained the cross sections of sub(152)Eu (Tsub(1/2)=12.4 g) and of sub(154)E (Tsub(1/2)=8.6 yr); they equal 11400+-1400 and 1530+-190 barn at E=0.0253 eV. The cross section of the sub(152)Eu absorption for the thermal spectrum (T=333 K) is determined by the activation method; it is 8900+-1200 barn

Frederick Soddy's invention of isotopes in 1911

International Nuclear Information System (INIS)

Attas, M.

2011-01-01

This paper describes the history of the invention of isotopes by Frederick Soddy in 1911. The idea of the nucleus had been conceived by a physicist, Ernest Rutherford. But it took a chemist, Frederick Soddy, to make chemical sense of the zoo of recently discovered radioactive elements, by inventing the idea of isotopes. He showed how one radioactive substance transformed itself spontaneously into another, following mathematical laws of exponential growth and decay. In his book The Chemistry of the Radio-Elements, Soddy compiled complete descriptions of the physical and chemical properties of each of the radioactive substances. He organized their sequences of transmutations by the.similarities in their chemical properties, so that the emanations, for example, were all side-by-side in a chart.

The ISOLDE Facility: Radioactive beams at CERN

CERN Multimedia

CERN. Geneva

2007-01-01

The Isope Separation On-Line (ISOL) technique evolved from chemical techniques used to separate radioactive isotopes off-line from irradiated "targets". The ISOL targets of today, used at e.g. ISOLDE, can be of many different types and in different phases but the isotopes are always delivered at very low energies making the technique ideal for study of ground state properties and collections for other applications such as solid state physics and medical physics. The possibility of accelerating these low energy beams for nuclear structure studies, and in the long term future for neutrino physics, is now being explored at first generation radioactive beam facilities. The upgrade towards HIE-ISOLDE aim to consolidate ISOLDE's position as a world leading radioactive nuclear beam facility and it will be a pre-cursor to a future all European ISOL facility, EURISOL, with order of magnitudes higher radioactive beam intensities and energies. Prerequisite knowledge and references: None

Isotopes Project

International Nuclear Information System (INIS)

Dairiki, J.M.; Browne, E.; Firestone, R.B.; Lederer, C.M.; Shirley, V.S.

1984-01-01

The Isotopes Project compiles and evaluates nuclear structure and decay data and disseminates these data to the scientific community. From 1940-1978 the Project had as its main objective the production of the Table of Isotopes. Since publication of the seventh (and last) edition in 1978, the group now coordinates its nuclear data evaluation efforts with those of other data centers via national and international nuclear data networks. The group is currently responsible for the evaluation of mass chains A = 167-194. All evaluated data are entered into the International Evaluated Nuclear Structure Data File (ENSDF) and are published in Nuclear Data Sheets. In addition to the evaluation effort, the Isotopes Project is responsible for production of the Radioactivity Handbook

Stable isotope enrichment: Current and future potential

International Nuclear Information System (INIS)

Tracy, J.G.; Aaron, W.S.

1992-01-01

Oak Ridge National Laboratory (ORNL) operates the Isotope Enrichment Facility for the purpose of providing enriched stable isotopes, selected radioactive isotopes (including the actinides), and isotope-related materials and services for use in various research applications. ORNL is responsible for isotope enrichment and the distribution of approximately 225 nongaseous stable isotopes from 50 multi-isotopic elements. Many enriched isotope products are of prime importance in the fabrication of nuclear targets and the subsequent production of special radionuclides. State-of-the-art techniques to achieve special isotopic, chemical, and physical requirements are performed at ORNL This report describes the status and capabilities of the Isotope Enrichment Facility and the Isotope Research Materials Laboratory as well as emphasizing potential advancements in enrichment capabilities

Stable isotope enrichment - current and future potential

International Nuclear Information System (INIS)

Tracy, J.G.; Aaron, W.S.

1993-01-01

Oak Ridge National Laboratory (ORNL) operates the Isotope Enrichment Facility for the purpose of providing enriched stable isotopes, selected radioactive isotopes (including the actinides), and isotope-related materials and services for use in various research applications. ORNL is responsible for isotope enrichment and the distribution of approximately 225 nongaseous stable isotopes from 50 multi-isotopic elements. Many enriched isotope products are of prime importance in the fabrication of nuclear targets and the subsequent production of special radionuclides. State-of-the-art techniques to achieve special isotopic, chemical, and physical requirements are performed at ORNL. This report describes the status and capabilities of the Isotope Enrichment Facility and the Isotope Research Materials Laboratory as well as emphasizing potential advancements in enrichment capabilities. (orig.)

Measurement of natural and {sup 137}Cs radioactivity concentrations at Izmit Bay (Marmara Sea), Turkey

Energy Technology Data Exchange (ETDEWEB)

Öksüz, İ., E-mail: ibrahim-ksz@yahoo.com; Güray, R. T., E-mail: tguray@kocaeli.edu.tr; Özkan, N., E-mail: nozkan@kocaeli.edu.tr; Yalçin, C., E-mail: caner.yalcin@kocaeli.edu.tr [Kocaeli University, Department of Physics, Umuttepe 41380, Kocaeli (Turkey); Ergül, H. A., E-mail: halim.ergul@kocaeli.edu.tr; Aksan, S., E-mail: serdar.aksan@kocaeli.edu.tr [Kocaeli University, Department of Biology, Umuttepe 41380, Kocaeli (Turkey)

2016-03-25

In order to determine the radioactivity level at Izmit Bay Marmara Sea, marine sediment samples were collected from five different locations. The radioactivity concentrations of naturally occurring {sup 238}U, {sup 232}Th and {sup 40}K isotopes and also that of an artificial isotope {sup 137}Cs were measured by using gamma-ray spectroscopy. Preliminary results show that the radioactivity concentrations of {sup 238}U and {sup 232}Th isotopes are lower than the average worldwide values while the radioactivity concentrations of the {sup 40}K are higher than the average worldwide value. A small amount of {sup 137}Cs contamination, which might be caused by the Chernobyl accident, was also detected.

Overview of the U.S. Department of Energy's Isotope Programs

Energy Technology Data Exchange (ETDEWEB)

Carty, J.

2004-10-05

This presentation provides an overview of the U.S. Department of Energy's Isotopes Program. The charter of the Isotope Programs covers the production and sale of radioactive and stable isotopes, associated byproducts, surplus materials, and related isotope services.

Treatment and storage of hydrogen isotopes

International Nuclear Information System (INIS)

Jung, H. S.; Lee, H. S.; An, D. H.; Kim, K. R.; Lee, S. H.; Choi, H. J.; Back, S. W.; Kang, H. S.; Eom, K. Y.; Lee, M. S.

2000-01-01

Storage of gaseous hydrogen isotopes in a cylinder is a well-established technology. However, Immobilization in the solid form is preferred for long-term storage of radioactive isotope gas because of the concern for leakage of the gas. The experimental thermodynamic p-c-T data show that Ti and U soak up hydrogen isotope gas at a temperature of a few hundred .deg. C and modest pressures. It was found that more hydrogen is dissolved in the metal than deuterium at constant pressure. Thus, the lighter isotope tends to be enriched in the solid phase

Radioactive waste management information for 1993 and record-to-date

International Nuclear Information System (INIS)

Taylor, K.A.

1994-07-01

This document presents detailed data, bar graphs, and pie charts on volume, radioactivity, isotopic identity, origin, and decay status of radioactive waste for the calendar year 1993. It also summarizes the radioactive waste data records compiled from 1952 to present for the Idaho National Engineering Laboratory (INEL). The data presented are from the INEL Radioactive Waste Management Information System

Radioactive waste management information for 1990 and record-to-date

International Nuclear Information System (INIS)

Litteer, D.L.; Peterson, C.N.; Sims, A.M.

1991-07-01

This document presents detailed data and graphics on volume, radioactivity, isotopic identity, origin, and decay status of radioactive waste for the calendar year 1990. It also summarizes the radioactive waste data records compiled from 1952 to present for the Idaho National Engineering Laboratory (INEL). The data presented are from the INEL Radioactive Waste Management Information System (RWMIS)

Production of radioactive molecular beams for CERN-ISOLDE

CERN Document Server

AUTHOR|(SzGeCERN)703149; Kröll, Thorsten

SOLDE, the Isotope Separation On-Line facility, at CERN is a leading facility for the production of beams of exotic radioactive isotopes. Currently over 1000 different isotopes with half lives down to milliseconds can be extracted with beam intensities of up to 10^11 ions per second. However, due to the reactive target environment not all isotopes are extractable in sufficient amounts. In this work the extraction of short lived carbon and boron isotopes is investigated. Therefore a variety of experimental and computanional techniques have been used.

Radioactivity of food products in the region of the ''Kozloduj'' atomic power station in the pre-exploitation period

International Nuclear Information System (INIS)

Jotov, M.; Petkov, T.; Zlatanova, R.; Boyadzhiev, A.

1976-01-01

The pre-exploitation status of the region of the ''Kozloduj'' atomic power stationand its torch zone, regarding the concentration of the biologically most dangerous artificial isotopes in the basic food products was determined. The tested foods were milk, meat, wheat, fish and grapes produced at the most important and basic production regions in the controled region. The radioactive isotope concentrations in the analyzed food produxts are reported. They will serve as a basis in assessing any eventual additional contamination of the region as a result of the work of the ''Kozloduj'' electric power station. (author)

Studies of neutron-deficient mendelevium isotopes at SHIP

Energy Technology Data Exchange (ETDEWEB)

Antalic, S.; Saro, S. [Comenius University, Department of Nuclear Physics and Biophysics, Bratislava (Slovakia); Hessberger, F.P.; Ackermann, D.; Heinz, S.; Kindler, B.; Kojouharov, I.; Lommel, B.; Mann, R. [GSI Helmholtzzentrum fuer Schwerionenforschung GmbH, Darmstadt (Germany); Hofmann, S. [GSI Helmholtzzentrum fuer Schwerionenforschung GmbH, Darmstadt (Germany); Goethe-Universitaet, Institut fuer Kernphysik, Frankfurt am Main (Germany); Kuusiniemi, P. [University of Oulu, Centre for Underground Physics in Pyhaesalmi (CUPP), Oulu (Finland); Leino, M. [University of Jyvaeskylae, Department of Physics, Jyvaeskylae (Finland)

2010-01-15

The radioactive decay of the isotopes {sup 247}Md, {sup 246}Md and their daughter products was investigated by means of {alpha}-{alpha} and {alpha}-{gamma} coincidence spectroscopy. The isotopes were produced using the fusion reaction {sup 40}Ar + {sup 209}Bi. Decay schemes are suggested for {sup 247}Md and {sup 243}Es. A new isomeric state in {sup 246}Md with a half-life of (4.4{+-}0.8) s was observed. Previous data of electron-capture delayed fission of {sup 246}Md and {sup 242}Es were confirmed. The probability for this decay branch in {sup 246}Md was measured to be P{sub ECDF}>0.10. The probability for electron-capture delayed fission in the case of {sup 242}Es was determined to be P{sub ECDF}=0.013{sup +0.012} {sub -0.007}. (orig.)

Coulomb excitation of radioactive {sup 79}Pb

Energy Technology Data Exchange (ETDEWEB)

Lister, C.J.; Blumenthal, D.; Davids, C.N. [and others

1995-08-01

The technical challenges expected in experiments with radioactive beams can already be explored by using ions produced in primary reactions. In addition, the re-excitation of these ions by Coulomb excitation allows a sensitive search for collective states that are well above the yrast line. We are building an experiment to study Coulomb excitation of radioactive ions which are separated from beam particles by the Fragment Mass Analyzer. An array of gamma detectors will be mounted at the focal plane to measure the gamma radiation following re-excitation. Five Compton-suppressed Ge detectors and five planar LEPS detectors will be used. The optimum experiment of this type appears to be the study of {sup 79}Rb following the {sup 24}Mg ({sup 58}Ni,3p) reaction. We calculate that about 5 x 10{sup 5} {sup 79}Rb nuclei/second will reach the excitation foil. This rubidium isotope was selected for study as it is strongly produced and is highly deformed, so easily re-excited. The use of a {sup 58}Ni re-excitation foil offers the best yields. After re-excitation the ions will be subsequently transported into a shielded beamdump to prevent the accumulation of activity.

Chemical investigations of isotope separation on line target units for carbon and nitrogen beams

CERN Document Server

Franberg, H; Gäggeler, H W; Köster, U

2006-01-01

Radioactive ion beams (RIBs) are of significant interest in a number of applications. Isotope separation on line (ISOL) facilities provide RIB with high beam intensities and good beam quality. An atom that is produced within the ISOL target will first diffuse out from the target material. During the effusion towards the transfer line and into the ion source the many contacts with the surrounding surfaces may cause unacceptable delays in the transport and, hence, losses of the shorter-lived isotopes. We performed systematic chemical investigations of adsorption in a temperature and concentration regime relevant for ISOL targets and ion source units, with regard to CO/sub x/ and NOmaterials are potential construction materials for the above-mentioned areas. Off-line and on-line tests have been performed using a gas thermochromatography setup with radioactive tracers. The experiments were performed at the production of tracers for atmospheric chemistry (PROTRAC) facility at the Paul Schener Institute in Villigen...

Understanding radioactive waste

International Nuclear Information System (INIS)

Murray, R.L.

1981-12-01

This document contains information on all aspects of radioactive wastes. Facts are presented about radioactive wastes simply, clearly and in an unbiased manner which makes the information readily accessible to the interested public. The contents are as follows: questions and concerns about wastes; atoms and chemistry; radioactivity; kinds of radiation; biological effects of radiation; radiation standards and protection; fission and fission products; the Manhattan Project; defense and development; uses of isotopes and radiation; classification of wastes; spent fuels from nuclear reactors; storage of spent fuel; reprocessing, recycling, and resources; uranium mill tailings; low-level wastes; transportation; methods of handling high-level nuclear wastes; project salt vault; multiple barrier approach; research on waste isolation; legal requiremnts; the national waste management program; societal aspects of radioactive wastes; perspectives; glossary; appendix A (scientific American articles); appendix B (reference material on wastes)

Understanding radioactive waste

Energy Technology Data Exchange (ETDEWEB)

Murray, R.L.

1981-12-01

This document contains information on all aspects of radioactive wastes. Facts are presented about radioactive wastes simply, clearly and in an unbiased manner which makes the information readily accessible to the interested public. The contents are as follows: questions and concerns about wastes; atoms and chemistry; radioactivity; kinds of radiation; biological effects of radiation; radiation standards and protection; fission and fission products; the Manhattan Project; defense and development; uses of isotopes and radiation; classification of wastes; spent fuels from nuclear reactors; storage of spent fuel; reprocessing, recycling, and resources; uranium mill tailings; low-level wastes; transportation; methods of handling high-level nuclear wastes; project salt vault; multiple barrier approach; research on waste isolation; legal requiremnts; the national waste management program; societal aspects of radioactive wastes; perspectives; glossary; appendix A (scientific American articles); appendix B (reference material on wastes). (ATT)

Radioactivity of neutron rich oxygen, fluorine and neon isotopes

International Nuclear Information System (INIS)

Reed, A.T.; Page, R.D.; Tarasov, O.

1999-01-01

The γ-radiation and neutrons emitted following the β-decays of 24 O, 25-27 F and 28-30 Ne have been measured. The nuclides were produced in the quasi-fragmentation of a 78 MeV/A 36 S beam, separated in-flight and identified through time-of-flight and energy loss measurements. The ions were stopped in a silicon detector system, which was used to detect the β-particles emitted in their subsequent radioactive decay. The coincident γ-rays were measured using four large Ge detectors mounted close to the implantation point and the neutrons were detected using forty-two 3 He proportional counters. The measured γ-ray energy spectra are compared with shell model calculations and, where available, the level energies are deduced from transfer reactions

Environmental isotope hydrology

International Nuclear Information System (INIS)

1973-01-01

Environmental isotope hydrology is a relatively new field of investigation based on isotopic variations observed in natural waters. These isotopic characteristics have been established over a broad space and time scale. They cannot be controlled by man, but can be observed and interpreted to gain valuable regional information on the origin, turnover and transit time of water in the system which often cannot be obtained by other techniques. The cost of such investigations is usually relatively small in comparison with the cost of classical hydrological studies. The main environmental isotopes of hydrological interest are the stable isotopes deuterium (hydrogen-2), carbon-13, oxygen-18, and the radioactive isotopes tritium (hydrogen-3) and carbon-14. Isotopes of hydrogen and oxygen are ideal geochemical tracers of water because their concentrations are usually not subject to change by interaction with the aquifer material. On the other hand, carbon compounds in groundwater may interact with the aquifer material, complicating the interpretation of carbon-14 data. A few other environmental isotopes such as 32 Si and 238 U/ 234 U have been proposed recently for hydrological purposes but their use has been quite limited until now and they will not be discussed here. (author)

Method of producing excited states of atomic nuclei

International Nuclear Information System (INIS)

Morita, M.; Morita, R.

1976-01-01

A method is claimed of producing excited states of atomic nuclei which comprises bombarding atoms with x rays or electrons, characterized in that (1) in the atoms selected to be produced in the excited state of their nuclei, (a) the difference between the nuclear excitation energy and the difference between the binding energies of adequately selected two electron orbits is small enough to introduce the nuclear excitation by electron transition, and (b) the system of the nucleus and the electrons in the case of ionizing an orbital electron in said atoms should satisfy the spin and parity conservation laws; and (2) the energy of the bombarding x rays or electrons should be larger than the binding energy of one of the said two electron orbits which is located at shorter distance from the atomic nucleus. According to the present invention, atomic nuclei can be excited in a relatively simple manner without requiring the use of large scale apparatus, equipment and production facilities, e.g., factories. It is also possible to produce radioactive substances or separate a particular isotope with an extremely high purity from a mixture of isotopes by utilizing nuclear excitation

Salinity dependent hydrogen isotope fractionation in alkenones produced by coastal and open ocean haptophyte algae

NARCIS (Netherlands)

M'boule, D.; Chivall, D.; Sinke-Schoen, D.; Sinninghe Damsté, J.S.; Schouten, S.; van der Meer, M.T.J.

2014-01-01

The hydrogen isotope fractionation in alkenones produced by haptophyte algae is a promising new proxy for paleosalinity reconstructions. To constrain and further develop this proxy the coastal haptophyte Isochrysis galbana and the open ocean haptophyte alga Emiliania huxleyi were cultured at

Viscous liquid barrier demonstration at the Brookhaven National Laboratory Linac Isotope Producer

International Nuclear Information System (INIS)

Heiser, J.H.; Sullivan, T.; Ludewig, H.; Brower, J.; North-Abbott, M.; Manchester, K.; Zaluski, M.; Penny, G.

2000-01-01

Groundwater monitoring has detected tritium ( 3 H) and 22 Na contamination down gradient from the Brookhaven LINAC Isotope Producer (BLIP), located at Brookhaven National Laboratory (BNL). Site characterization studies indicate that the BLIP is the source of contamination. The highest measured values for 3 H were 52,400 pCi/L recorded less than 100 feet south (down gradient) of the BLIP facility. The BLIP produces radioisotopes that are crucial in nuclear medicine for both research and clinical use. The BLIP also supports research on diagnostic and therapeutic radiopharmaceuticals. During operation a proton beam impinges a target (typically salts encapsulated in stainless steel) to produce the required radioisotopes. The proton beam is completely absorbed prior to reaching the soils surrounding the target shaft. However, secondary neutrons are produced that reach the soil causing activation products to form. Among the longer-lived isotopes of concern are tritium and 22 Na. Both of these isotopes have the potential to negatively impact the groundwater below the BLIP. Several corrective actions have been implemented at the BLIP facility in response to tritium detection in the groundwater. The first actions were to improve surface water management (e.g. storm water down spouts) and the installation of a gunite cap around the BLIP facility. These measures are designed to minimize water flow through the activated soils in the vicinity of BLIP. In conjunction with these improvements, BNL is installing a close-proximity subsurface barrier in the activated soils beneath the BLIP facility. The barrier will prevent water migration through the activated soil zone as well as prevent activation product migration out of the zone. To minimize impacts on the operation of the BLIP requires in-situ barrier installation using low energy techniques that will not disturb the alignment of the BLIP or nearby accelerator beams. BNL chose an innovative barrier technology termed Viscous

A hydrochemical and isotopic case study around a near surface radioactive waste disposal

International Nuclear Information System (INIS)

Szanto, Zs.; Svingor, E.; Futo, I.; Palcsu, L.; Molnar, M.; Rinyu, L.

2007-01-01

As part of the site characterisation program for the near surface radioactive waste treatment and disposal facility (RWTDF) at Puespoekszilagy, Hungary, water quality and environmental isotope investigations have been carried out. Water samples for major ion chemistry, tritium, 14 C and stable isotope ratio measurements (δ 18 O, δD, δ 34 S, δ 13 C) were taken quarterly from the observation wells, the streams and the precipitation during the period 1999-2001. The chemical composition of groundwaters presented a continuous transition from waters situated on one side to waters on the top and on the other slope of the disposal suggesting the mixing of the three hydrochemical ''endmembers''. Most of δD and δ 18 O data were situated between GMWL and LMWL (δD = 7.2 x δ 18 O - 1 permille) with Oligocene aquifer presenting recharge of Pleistocene origin and water on the top and the gentle slope of the hill presenting recharge of Holocene origin. δ 34 S values of dissolved sulphates varied in a wide range (-14.2 permille to +5.4 permille). The tritium in precipitation varied between 4.4 and 18.1 TU with an annual weighted average of 10 ± 0.3 TU. The streams showed larger fluctuations than the wells, but the changes of δ 18 O, δD and T were small compared to those in precipitation (showing seasonal variation). Stable isotope, tritium and radiocarbon data proved that the replenishment of groundwater is slow on the steeper side and the direction of water movement is toward the gentle slope of the hill. It was judged that this path is the one that is most likely to give rise to high doses and, therefore, was used in the hydrological modelling of the safety assessment that followed the present work. The possibility that there may also be transport through the unsaturated zone and systems of perched water tables in layers 1 and 2 to both the Szilagyi and Nemedi streams cannot be excluded; the transport along these pathways is likely to be intermittent. (orig.)

Production of radioactive molecular beams for CERN-ISOLDE

Energy Technology Data Exchange (ETDEWEB)

Seiffert, Christoph

2015-06-15

ISOLDE, the Isotope Separation On-Line facility, at CERN is a leading facility for the production of beams of exotic radioactive isotopes. Currently over 1000 different isotopes with half lives down to milliseconds can be extracted with beam intensities of up to 10{sup 11} ions per second. However, due to the reactive target environment not all isotopes are extractable in sufficient amounts. In this work the extraction of short lived carbon and boron isotopes is investigated. Therefore a variety of experimental and computational techniques have been used.

Radioactive inventory in structural materials of ET-R R-1 reactor and its implication on decommissioning.

Energy Technology Data Exchange (ETDEWEB)

Elkady, A; Amin, E [National center for nuclear safety and radiation control, atomic energy authority, Cairo, (Egypt)

1995-10-01

A plan for decommissioning of ET-R R-1 reactor should include estimation of radioactivity in structural materials. The inventory will help in assessing the radiological consequences decommissioning. Conservative calculations have been made to evaluate the activity of the long lived isotopes which can be produced by neutron activation. The materials which are present in significant quantities in the reactor structural materials are aluminium, cast iron, graphite, ordinary and iron shot concrete. The radioactivity of each component is dependent not only upon the major elements, but also on the concentration of the trace elements. The main radioactive inventory are expected to be from Co-60 and Fe-55 which are present in aluminium as trace elements in larger quantities in other construction materials. 2 figs., 4 tabs.

Studies on the behaviour of some radioactive pollutants into soil-fresh water environment

International Nuclear Information System (INIS)

Sayed, M.S.

1989-01-01

The overwhelming increase in the use of nuclear power plants comes to cover many purposes, such as generating of electricity, desalination of sea water, and producing radioactive isotopes in large quantities. There is no doubt that the continuous increase in the production of radioisotope, presents an outstanding potential health hazard to man and its environment. Many radio-nuclide wastes, may be released to the environment from nuclear research reactors, hospitals, universities etc in large quantities and low radioactive level which can contaminate drinking and underground water, plants, animals and air. The present work includes introduction which is a literature survey of uses of natural minerals and clays in the treatment of low level radioactive wastes and the different chemical methods used for their treatment e.g. co-participation, adsorption chromatography, ion exchange , solvent extraction, coagulation and flocculation etc

Electron linac for medical isotope production with improved energy efficiency and isotope recovery

Science.gov (United States)

Noonan, John; Walters, Dean; Virgo, Matt; Lewellen, John

2015-09-08

A method and isotope linac system are provided for producing radio-isotopes and for recovering isotopes. The isotope linac is an energy recovery linac (ERL) with an electron beam being transmitted through an isotope-producing target. The electron beam energy is recollected and re-injected into an accelerating structure. The ERL provides improved efficiency with reduced power requirements and provides improved thermal management of an isotope target and an electron-to-x-ray converter.

Alternative solutions for the disposal of radioactive wastes

International Nuclear Information System (INIS)

Ramsey, R.W. Jr.

1976-01-01

Besides outlining the possibility of dispatching concentrated highly radioactive waste by rockets into space, or of transmuting long-lived isotopes by nuclear reactions into short-lived ones, the author discusses further alternatives for the disposal of radioactive wastes, especially the storage in geologic formations. (HR/LN) [de

New Isotope Analysis Method: Atom Trap Mass Spectrometry

International Nuclear Information System (INIS)

Ko, Kwang Hoon; Park, Hyun Min; Han, Jae Min; Kim, Taek Soo; Cha, Yong Ho; Lim, Gwon; Jeong, Do Young

2011-01-01

Trace isotope analysis has been an important role in science, archaeological dating, geology, biology and nuclear industry. Some fission products such as Sr-90, Cs-135 and Kr-85 can be released to the environment when nuclear accident occurs and the reprocessing factory operates. Thus, the analysis of artificially produced radioactive isotopes has been of interest in nuclear industry. But it is difficult to detect them due to low natural abundance less then 10 -10 . In general, radio-chemical method has been applied to detect ultra-trace radio isotopes. But this method has disadvantages of long measurement time for long lived radioisotopes and toxic chemical process for the purification. The Accelerator Mass Spectrometer has high isotope selectivity, but the system is huge and its selectivity is affected by isobars. The laser based method, such as RIMS (Resonance Ionization Mass Spectrometry) has the advantage of isobar-effect free characteristics. But the system size is still huge for high isotope selective system. Recently, ATTA (Atom Trap Trace Analysis) has been successfully applied to detect ultra-trace isotope, Kr-81 and Kr-85. ATTA is the isobar-effect free detection with high isotope selectivity and the system size is small. However, it requires steady atomic beam source during detection, and is not allowed simultaneous detection of several isotopes. In this presentation, we introduce new isotope detection method which is a coupled method of Atom Trap Mass Spectrometry (ATMS). We expect that it can overcome the disadvantage of ATTA while it has both advantages of ATTA and mass spectrometer. The basic concept and the system design will be presented. In addition, the experimental status of ATMS will also be presented

Environmental isotopes assist in the site assessment of Vaalputs radioactive waste disposal facility

International Nuclear Information System (INIS)

Verhagen, B.T.; Levin, M.

1986-01-01

The first South African nuclear waste disposal facility is to be sited in an arid environment with an average annual rainfall of about 78mm. The ground water might therefore be virtually stationary, making the geohydrology of the area crucial in the assessment of radionuclide dispersal difficult to study with standard hydraulic methods. Environmental isotopes, which label the water itself and some of its dissolved constituents are able to give synoptic information about the ground water; from this, some projections about future mobility can be made. Tritium profiles in the unsaturated zone show the limited extent of rain water infiltration, which generally extends down to 3-4 metres, with sporadic evidence of deeper penetration through cracks and rootholes in the thick clay cover. Soil moisture therefore seems to occur in tightly bound and more mobile components. This is confirmed by occasionally measurable tritium observed in the saturated zone. Radiocarbon in the ground water cannot be simply interpreted on account of the nature of the granite aquifer. Although suggesting ages of several thousands of years, radiocarbon proves that the water is not 'fossil' or derived from the last pluvial period, postulated to have occurred some 12 000 years ago. Recharge appears to be more ongoing and to occur periodically and locally as a result of outliers within the present climatological regime. Regional movement of ground water is however very limited, as spatial variations seen in the radiocarbon data of the ground water are non-systematic. These conclusions are supported by the distribution of the non-radioactive isotopes, such as oxygen-18

Isotope distribution program at the Oak Ridge National Laboratory with emphasis on medical isotopes

International Nuclear Information System (INIS)

Adair, H.L.

1987-01-01

The Isotope Distribution Program (IDP) is a group of individual activities with separate and diverse DOE sponsors which share the common mission of the production and distribution of isotope products and the performance of isotope-related services. Its basic mission is to provide isotope products and associated services to the user community by utilizing government-owned facilities that are excess to the primary mission of the DOE. The IDP is in its 41st year of operation. Initially, the program provided research quantities of radioactive materials, and through the 1950's it was the major supplier of radioisotopes for both research and commercial application. Distribution of enriched stable isotopes began in 1954. This paper discusses the use of radioisotopes in medicine and the role that ORNL plays in this field

Nuclear chemistry research and spectroscopy with radioactive sources. Twenty-second annual progress report, February 1, 1986-January 31, 1987

International Nuclear Information System (INIS)

Fink, R.W.

1986-01-01

The nuclear chemistry group in the School of Chemistry continues investigations of radioactive decay of nuclei far from stability under this DOE contract. These nuclei are produced with heavy ions from the Holifield Heavy Ion Research Facility (HHIRF) and studied on-line with the University Isotope Separator at Oak Ridge (UNISOR). Radioactive decay represents a unique method for the population of low-energy, low-spin structures in nuclei, and new phenomena which do not occur near stability can be explored. Our research interest encompasses three aspects of nuclear structure: (1) nuclear spectroscopy with detailed γγt, e - γt, Xγt, αγt multiparameter coincidence spectrometry; (2) measurements of single γ-ray angular distributions and magnetic moments of mass separated low-temperature oriented nuclei, using the helium dilution refrigerator ''ORIENT'' being installed on-line to the isotope separator; and (3) on-line laser hyperfine structure (hfs) and isotope shift measurements for determination of nuclear quadrupole moments, nuclear spins, and changes in mean nuclear charge radii as a means of revealing systematic shape changes in nuclei. 35 refs., 8 figs., 1 tab

Travel Times of Water Derived from Three Naturally Occurring Cosmogenic Radioactive Isotopes

Science.gov (United States)

Visser, Ate; Thaw, Melissa; Deinhart, Amanda; Bibby, Richard; Esser, Brad

2017-04-01

Hydrological travel times are studied on scales that span six orders of magnitude, from daily event water in stream flow to pre-Holocene groundwater in wells. Groundwater vulnerability to contamination, groundwater surface water interactions and catchment response are often focused on "modern" water that recharged after the introduction of anthropogenic tritium in precipitation in 1953. Shorter residence times are expected in smaller catchments, resulting in immediate vulnerability to contamination. We studied a small (4.6 km2) alpine (1660-2117 m) catchment in a Mediterranean climate (8 ˚ C, 1200 mm/yr) in the California Sierra Nevada to assess subsurface storage and investigate the response to the recent California drought. We analyzed a combination of three cosmogenic radioactive isotopes with half-lives varying from 87 days (sulfur-35), 2.6 years (sodium-22) to 12.3 years (tritium) in precipitation and stream samples. Tritium samples (1 L) are analyzed by noble gas mass spectrometry after helium-3 accumulation. Samples for sulfur-35 and sodium-22 are collected by processing 20-1000 L of water through an anion and cation exchange column in-situ. Sulfur-35 is analyzed by liquid scintillation counting after chemical purification and precipitation. Sodium-22 is analyzed by gamma counting after eluting the cations into a 4L Marinelli beaker. Monthly collected precipitation samples show variability of deposition rate for tritium and sulfur-35. Sodium-22 levels in cumulative yearly precipitation samples are consistent with recent studies in the US and Japan. The observed variability of deposition rates complicates direct estimation of stream water age fractions. The level and variability of tritium in monthly stream samples indicate a mean residence time on the order of 10 years and only small contributions of younger water during high flow conditions. Estimates of subsurface storage are in agreement with estimates from geophysical studies. Detections of sodium-22

The A.B.Cs of isotope hydrology

International Nuclear Information System (INIS)

Maduabuchi, C.

2000-01-01

The steady growth in world population coupled with the extension of irrigated agriculture and accelerated industrial development and other economic activities have put tremendous stress on the quantity and quality aspects of surface and groundwater resources the world over. The situation calls for necessary monitoring mechanism to safeguard these renewable but potentially depletable resources. A proper understanding of water resources systems is a prerequisite to their sustainable development. This informed the application of isotope techniques in hydrology as they provide vital information that are not readily obtainable from the classical hydrological techniques. These include issues relating to origin and history of groundwater, recharge estimates, vulnerability of aquifers to pollution, mixing proportion of component flows and study of geothermal systems amongst others. Maximum benefits are derived from the application of isotope techniques when they are complemented with conventional techniques in an integrated manner. The paper discusses the basic concepts which include configuration of the nucleus of the atom, isotopes, radioactivity and radioactive decay law. It further explains the occurrence of environmental isotopes including their measurement in natural compounds and the general application of isotopes in water resources development and management

The beam diagnostic instruments in Beijing radioactive ion-beam facilities isotope separator on-line

International Nuclear Information System (INIS)

Ma, Y.; Cui, B.; Ma, R.; Tang, B.; Chen, L.; Huang, Q.; Jiang, W.

2014-01-01

The beam diagnostic instruments for Beijing Radioactive Ion-beam Facilities Isotope Separator On-Line are introduced [B. Q. Cui, Z. H. Peng, Y. J. Ma, R. G. Ma, B. Tang, T. Zhang, and W. S. Jiang, Nucl. Instrum. Methods 266, 4113 (2008); T. J. Zhang, X. L. Guan, and B. Q. Cui, in Proceedings of APAC 2004, Gyeongju, Korea, 2004, http://www.jacow.org , p. 267]. For low intensity ion beam [30–300 keV/1 pA–10 μA], the beam profile monitor, the emittance measurement unit, and the analyzing slit will be installed. For the primary proton beam [100 MeV/200 μA], the beam profile scanner will be installed. For identification of the nuclide, a beam identification unit will be installed. The details of prototype of the beam diagnostic units and some experiment results will be described in this article

Stable isotope analysis of the human body. What isotopes in our tissue can reveal and what not; Stabilisotopenanalysen am Menschen. Was die Isotopie unseres Koerpergewebes ueber uns verraet- und was nicht

Energy Technology Data Exchange (ETDEWEB)

Goerger, Marlene [Technische Univ. Darmstadt (Germany)

2016-07-01

Most isotopes in the natural environment are stable but there are radioactive isotopes. Premordial radionuclides are nuclides that exist since the development of the earth crust. Cosmogenic radionuclides are generated due to cosmic radiation (protons, electrons, ionized atoms) - for instance C-14. Radiogenic nuclides are daughter products of radioactive nuclei. Anthropogenic radionuclides are generated due to human activities. Deviations from a ''normal'' isotope distribution are used for environmental impact analysis and forensic purposes. The human provenance project was stopped.

A nuclear physics program at the Rare Isotope Beams Accelerator Facility in Korea

Directory of Open Access Journals (Sweden)

Chang-Bum Moon

2014-02-01

Full Text Available This paper outlines the new physics possibilities that fall within the field of nuclear structure and astrophysics based on experiments with radioactive ion beams at the future Rare Isotope Beams Accelerator facility in Korea. This ambitious multi-beam facility has both an Isotope Separation On Line (ISOL and fragmentation capability to produce rare isotopes beams (RIBs and will be capable of producing and accelerating beams of wide range mass of nuclides with energies of a few to hundreds MeV per nucleon. The large dynamic range of reaccelerated RIBs will allow the optimization in each nuclear reaction case with respect to cross section and channel opening. The low energy RIBs around Coulomb barrier offer nuclear reactions such as elastic resonance scatterings, one or two particle transfers, Coulomb multiple-excitations, fusion-evaporations, and direct capture reactions for the study of the very neutron-rich and proton-rich nuclides. In contrast, the high energy RIBs produced by in-flight fragmentation with reaccelerated ions from the ISOL enable to explore the study of neutron drip lines in intermediate mass regions. The proposed studies aim at investigating the exotic nuclei near and beyond the nucleon drip lines, and to explore how nuclear many-body systems change in such extreme regions by addressing the following topics: the evolution of shell structure in areas of extreme proton to neutron imbalance; the study of the weak interaction in exotic decay schemes such as beta-delayed two-neutron or two-proton emission; the change of isospin symmetry in isobaric mirror nuclei at the drip lines; two protons or two neutrons radioactivity beyond the drip lines; the role of the continuum states including resonant states above the particle-decay threshold in exotic nuclei; and the effects of nuclear reaction rates triggered by the unbound proton-rich nuclei on nuclear astrophysical processes.

Proceedings of the International conference on radioecology and environmental radioactivity

International Nuclear Information System (INIS)

2008-01-01

The conference contains 404 presentations on: 1) Emergency preparedness and rehabilitation with emphasis on radiation and radioactivity determination and monitoring, protection and contamination and pollution. 2) TNORM/NORM including radon with focus on radioactivity in the environmental and isotope evaluation. 3) Radioecology and speciation including arctic radioecology, focusing on accidents, radiation and radioactivity effects, nuclear waste disposal, handling, impacts, safety and risks, pollution and its sources, accumulation of isotopes and various medical aspects. 4) Risk assessment with emphasis on the environmental and ecological aspects, modeling, recommendations and international cooperation and discussion of the effects of climatic changes. 5) Radiation in society. 6) Environmental protection with focus on radionuclide studies, radiation effects and protection measures, isotope accumulation effects, nuclide distribution, migration and pollution and effects and handling of nuclear accidents. The global aspects of the topics are evident and there are discussions on non-ionizing and ionizing radiation effect, various simulation problems and public and general health aspects (tk)

Travel in the depth of radioactivity; Voyage au coeur de la radioactivite

Energy Technology Data Exchange (ETDEWEB)

NONE

1996-09-01

This educational booklet gives a general presentation of radioactivity: origin of natural radioactivity, characteristics of atoms and isotopes, the radioactivity phenomenon, its decay and measurement units, the radiations and their use in medicine, industry, agriculture and food industry, biology etc.. (J.S.)

Short-lived radionuclides produced on the ORNL 86-inch cyclotron and High-Flux Isotope Reactor

International Nuclear Information System (INIS)

Lamb, E.

1985-01-01

The production of short-lived radionuclides at ORNL includes the preparation of target materials, irradiation on the 86-in. cyclotron and in the High Flux Isotope Reactor (HFIR), and chemical processing to recover and purify the product radionuclides. In some cases the target materials are highly enriched stable isotopes separated on the ORNL calutrons. High-purity 123 I has been produced on the 86-in. cyclotron by irradiating an enriched target of 123 Te in a proton beam. Research on calutron separations has led to a 123 Te product with lower concentrations of 124 Te and 126 Te and, consequently to lower concentrations of the unwanted radionuclides, 124 I and 126 I, in the 123 I product. The 86-in. cyclotron accelerates a beam of protons only but is unique in providing the highest available beam current of 1500 μA at 21 MeV. This beam current produces relatively large quantities of radionuclides such as 123 I and 67 Ga

The method for production of high purity carrier free ortophosphoric acid labeled with isotopes Phosphorus-32 and Phosphorus-33

International Nuclear Information System (INIS)

Abdukayumov, M.N.; Abdusalyamov, A.N.; Chistyakov, P.G.; Yuldashev, B.S.

2001-01-01

Extensive application for various radioactive isotopes was found in an extremity of the 20-Th century in a science and production. Labeled compounds are used with growing effectiveness in a molecular biology, gene engineering, medicine and other areas. Phosphorus-32 and Phosphorus-33 isotopes as a different labeled compounds that are used mainly in molecular biology are produced at the Radiopreparat enterprise of the Institute of Nuclear Physics of Academy of Sciences of Uzbekistan Republic. The quality of labeled preparations is very high. The specifications for above mentioned preparations corresponds to demands most of customers in different countries. P-32 or P-33 labeled orthophosphoric acid has high radiochemical purity (more than 99 %) and specific radioactivity close to theoretical. Orthophosphoric acid prepared by the described above method has radiochemical purity about 95 % and output of the target product 99%

Development of pharmaceuticals with radioactive rhenium for cancer therapy. Production of {sup 186}Re and {sup 188}Re, synthesis of labeled compounds and their biodistributions

Energy Technology Data Exchange (ETDEWEB)

NONE

1998-03-01

Production of the radioactive rhenium isotopes {sup 186}Re and {sup 188}Re, and synthesis of their labeled compounds have been studied together with the biodistributions of the compounds. This work was carried out by the Working Group on Radioactive Rhenium, consisting of researchers of JAERI and some universities, in the Subcommittee for Production and Radiolabeling under the Consultative Committee of Research on Radioisotopes. For {sup 186}Re, production methods by the {sup 185}Re(n,{gamma}){sup 186}Re reaction in a reactor and by the {sup 186}W(p,n){sup 186}Re reaction with an accelerator, which can produce nocarrier-added {sup 186}Re, have been established. For {sup 188}Re, a production method by the double neutron capture reaction of {sup 186}W, which produces a {sup 188}W/{sup 188}Re generator, has been established. For labeling of bisphosphonate, DMSA, DTPA, DADS, aminomethylenephosphonate and some monoclonal antibodies with the radioactive rhenium isotopes, the optimum conditions, including pH, the amounts of reagents and so on, have been determined for each compound. The biodistributions of each of the labeled compounds in mice have been also obtained. (author)

Using radioactivity

International Nuclear Information System (INIS)

1982-10-01

The leaflet discusses the following: radioactivity; radioisotopes; uses of ionising radiations; radioactivity from (a) naturally occurring radioactive elements, and (b) artificially produced radioisotopes; uses of radioactivity in medicine, (a) clinical diagnostic, (b) therapeutic (c) sterilization of medical equipment and materials; environmental uses as tracers; industrial applications, e.g. tracers and radiography; ensuring safety. (U.K.)

Disposal method of radioactive wastes

International Nuclear Information System (INIS)

Uetake, Naoto; Fukazawa, Tetsuo.

1986-01-01

Purpose: To improve the safety of underground disposal of radioactive wastes for a long period of time by surrounding the periphery of the radioactive wastes with materials that can inhibit the migration of radioactive nuclides and are physically and chemically stable. Method: Hardening products prepared from a water-hardenable calcium silicate compound and an aqueous solution of alkali silicate have compression strength as comparable with that of concretes, high water tightness and adsorbing property to radioactive isotopes such as cobalt similar to that of concretes and they also show adsorption to cesium which is not adsorbed to concretes. Further, the kneaded slurry thereof is excellent in the workability and can be poured even into narrow gaps. Accordingly, by alternately charging granular radioactive wastes and this slurry before hardening into the ground, the radioactive wastes can be put to underground disposal stably with simple procedures. (Kamimura, M.)

Beneficial uses and production of isotopes

CERN Document Server

2001-01-01

Isotopes, radioactive and stable, are used worldwide in various applications related to medical diagnosis or care, industry and scientific research. More than fifty countries have isotope production or separation facilities operated for domestic supply, and sometimes for international markets. This publication provides up-to-date information on the current status of, and trends in, isotope uses and production. It also presents key issues, conclusions and recommendations, which will be of interest to policy makers in governmental bodies, scientists and industrial actors in the field.

Study of reactions of isotopic exchange of trans-zeatin with tritium

International Nuclear Information System (INIS)

Sidorov, G.V.; Myasoedov, N.F.

2006-01-01

Reactions of isotopic exchange of trans-zeatin with high-radioactive tritium water, with gaseous tritium in solution and solid-phase catalytic hydrogenation are studied to prepare trans-zeatin and dihydrozeatin labelled with tritium. It is shown that reaction of isotopic exchange of trans-zeatin with gaseous tritium both in solutions and without solvents at 160 Deg C and above leads to practically total hydrogenation of initial compound with formation of dihydrozeatin labelled with tritium. Isotopic exchange with tritium water permits to prepare zeatin labelled with tritium with 67 % yield and specific radioactivity 0.68 PBq/mol. It is determined that in the case of solid-phase isotopic exchange within 150-155 Deg C temperature interval both dihydrozeatin and trans-zeatin labelled with tritium are formed [ru

Low-energy Coulomb excitation of neutron-rich zinc isotopes

CERN Document Server

Van de Walle, J; Behrens, T; Bildstein, V; Blazhev, A; Cederkäll, J; Clément, E; Cocolios, T E; Davinson, T; Delahaye, P; Eberth, J; Ekström, A; Fedorov, D V; Fedosseev, V; Fraile, L M; Franchoo, S; Gernhäuser, R; Georgiev, G; Habs, D; Heyde, K; Huber, G; Huyse, M; Ibrahim, F; Ivanov, O; Iwanicki, J; Jolie, J; Kester, O; Köster, U; Kröll, T; Krücken, R; Lauer, M; Lisetskiy, A F; Lutter, R; Marsh, B A; Mayet, P; Niedermaier, O; Pantea, M; Raabe, R; Reiter, P; Sawicka, M; Scheit, H; Schrieder, G; Schwalm, D; Seliverstov, M D; Sieber, T; Sletten, G; Smirnova, N; Stanoiu, M; Stefanescu, I; Thomas, J C; Valiente-Dobón, J J; Van Duppen, P; Verney, D; Voulot, D; Warr, N; Weisshaar, D; Wenander, F; Wolf, B H; Zielinska, M

2009-01-01

At the radioactive ion beam facility REX-ISOLDE, neutron-rich zinc isotopes were investigated using low-energy Coulomb excitation. These experiments have resulted in B(E2,20) values in 74-80Zn, B(E2,42) values in 74,76Zn and the determination of the energy of the first excited 2 states in 78,80Zn. The zinc isotopes were produced by high-energy proton- (A=74,76,80) and neutron- (A=78) induced fission of 238U, combined with selective laser ionization and mass separation. The isobaric beam was postaccelerated by the REX linear accelerator and Coulomb excitation was induced on a thin secondary target, which was surrounded by the MINIBALL germanium detector array. In this work, it is shown how the selective laser ionization can be used to deal with the considerable isobaric beam contamination and how a reliable normalization of the experiment can be achieved. The results for zinc isotopes and the N=50 isotones are compared to collective model predictions and state-of-the-art large-scale shell-model calculations, i...

Complete isotopic distributions of fragments produced in transfer- and fusion-induced reactions

International Nuclear Information System (INIS)

Delaune, O.; Caamano, M.; Farget, F.; Tarasov, O. B.; Derkx, X.; Schmidt, K. H.; Audouin, L.; Amthor, A. M.; Bacri, C. O.; Barreau, G.; Bastin, B.; Bazin, D.; Benlliure, J.; Blank, B.; Caceres, L.; Casarejos, E.; Fernandez-Dominguez, B.; Gaudefroy, L.; Golabek, C.; Grevy, S.; Jurado, B.; Kamalou, O.; Lemasson, A.; Lukyanov, S. M.; Mittig, W.; Morrissey, D. J.; Navin, A.; Pereira, J.; Perrot, L.; Rejmund, M.; Roger, T.; Saint-Laurent, M. G.; Savajols, H.; Schmitt, C.; Sherrill, B. M.; Stodel, C.; Thomas, J. C.; Villari, A. C. C.

2013-01-01

Two fission experiments have been performed at GANIL using 238 U beams at different energies and light targets. Different fissioning systems were produced with centre of mass energies from 10 to 240 MeV and their decay by fission was investigated with GANIL spectrometers. Fission-fragment isotopic distributions have been obtained. The evolution with impinging energy of their properties, the neutron excess and the width of the neutron-number distributions, gives important insights into the dynamics of the fusion-fission mechanism. (authors)

Radioactivity of Consumer Products

Science.gov (United States)

Peterson, David; Jokisch, Derek; Fulmer, Philip

2006-11-01

A variety of consumer products and household items contain varying amounts of radioactivity. Examples of these items include: FiestaWare and similar glazed china, salt substitute, bananas, brazil nuts, lantern mantles, smoke detectors and depression glass. Many of these items contain natural sources of radioactivity such as Uranium, Thorium, Radium and Potassium. A few contain man-made sources like Americium. This presentation will detail the sources and relative radioactivity of these items (including demonstrations). Further, measurements of the isotopic ratios of Uranium-235 and Uranium-238 in several pieces of china will be compared to historical uses of natural and depleted Uranium. Finally, the presenters will discuss radiation safety as it pertains to the use of these items.

Use of environmental radioactive isotopes in geothermal prospecting

International Nuclear Information System (INIS)

Balcazar, M.; Lopez M, A.; Huerta, M.; Flores R, J. H.; Pena, P.

2010-10-01

Oil resources decrease and environmental impact of burning fossil fuels support the use of alternative energies around the world. By far nuclear energy is the alternative which can supply huge amount of clean energy. Mexico has two nuclear units and has also explored and exploited the use of other complementary renewal energies, as wind and geothermal. Mexico is the third geothermal-energy producer in the world with an installed capacity of 960 MW and is planning the installation of 146 MW for the period 2010-2011, according to information of the Mexican Federal Electricity Board. This paper presents a study case, whose goal is to look for areas where the heat source can be located in geothermal energy fields under prospecting. The method consist in detecting a natural radioactive tracer, which is transported to the earth surface by geo-gases, generated close to the heat source, revealing areas of high permeability properties and open active fractures. Those areas are cross correlated to other resistivity, gravimetric and magnetic geophysical parameters in the geothermal filed to better define the heat source in the field. (Author)

A two-zone cosmic ray propagation model and its implication of the surviving fraction of radioactive cosmic ray isotopes

International Nuclear Information System (INIS)

Simon, M.; Scherzer, R.; Enge, W.

1977-01-01

In cosmic ray propagation calculations one can usually assume a homogeneous distribution of interstellar matter. The crucial astrophysical parameters in these models are: The path length distribution, the age of the cosmic ray particles and the interstellar matter density. These values are interrelated. The surviving fraction of radioactive cosmic ray isotopes is often used to determine a mean matter density of that region, where the cosmic ray particles may mainly reside. Using a Monte Carlo Propagation Program we calculated the change in the surviving fraction quantitatively assuming a region around the sources with higher matter density. (author)

Cold valleys in the radioactive decay of 248-254Cf isotopes

International Nuclear Information System (INIS)

Biju, R.K.; Sahadevan, Sabina; Santhosh, K.P.; Joseph, Antony

2008-01-01

Based on the concept of cold valley in cold fission and fusion, we have investigated the cluster decay process in 248-254 Cf isotopes. In addition to alpha particle minima, other deep minima occur for S, Ar and Ca clusters. It is found that inclusion of proximity potential does not change the position of minima but minima become deeper. Taking Coulomb and proximity potential as interacting barrier for post-scission region, we computed half-lives and other characteristics for various clusters from these parents. Our study reveals that these parents are stable against light clusters and unstable against heavy clusters. Computed half-lives for alpha decay agree with experimental values within two orders of magnitude. The most probable clusters from these parents are predicted to be 46 Ar, 48,50 Ca which indicate the role of doubly or near doubly magic clusters in cluster radioactivity. Odd A clusters are found to be favorable for emission from odd A parents. Cluster decay model is extended to symmetric region and it is found that symmetric fission is also probable which stresses the role of doubly or near doubly magic 132 Sn nuclei. Geiger-Nuttal plots were studied for various clusters and are found to be linear with varying slopes and intercepts. (author)

Determination of the isotopic ratio 234 U/238 U and 235 U/238 U in uranium commercial reagents by alpha spectroscopy

International Nuclear Information System (INIS)

Iturbe G, J.L.

1990-02-01

In this work the determination of the isotope ratio 234 U/ 238 U and 235 U/ 238 U obtained by means of the alpha spectroscopy technique in uranium reagents of commercial marks is presented. The analyzed uranium reagents were: UO 2 (*) nuclear purity, UO 3 (*) poly-science, metallic uranium, uranyl nitrate and uranyl acetate Merck, uranyl acetate and uranyl nitrate Baker, uranyl nitrate (*) of the Refinement and Conversion Department of the ININ, uranyl acetate (*) Medi-Lab Sigma of Mexico and uranyl nitrate Em Science. The obtained results show that the reagents that are suitable with asterisk (*) are in radioactive balance among the one 234 U/ 238 U, since the obtained value went near to the unit. In the case of the isotope ratio 235 U/ 238 U the near value was also obtained the one that marks the literature that is to say 0.04347, what indicates that these reagents contain the isotope of 235 U in the percentage found in the nature of 0.71%. The other reagents are in radioactive imbalance among the 234 U/ 238 U, the found values fluctuated between 0.4187 and 0.1677, and for the quotient of activities 235 U/ 238 U its were of 0.0226, and the lowest of 0.01084. Also in these reagents it was at the 236 U as impurity. The isotope of 236 U is an isotope produced artificially, for what is supposed that the reagents that are in radioactive imbalance were synthesized starting from irradiated fuel. (Author)

Thermal treatment of organic radioactive waste

International Nuclear Information System (INIS)

Chrubasik, A.; Stich, W.

1993-01-01

The organic radioactive waste which is generated in nuclear and isotope facilities (power plants, research centers and other) must be treated in order to achieve a waste form suitable for long term storage and disposal. Therefore the resulting waste treatment products should be stable under influence of temperature, time, radioactivity, chemical and biological activity. Another reason for the treatment of organic waste is the volume reduction with respect to the storage costs. For different kinds of waste, different treatment technologies have been developed and some are now used in industrial scale. The paper gives process descriptions for the treatment of solid organic radioactive waste of low beta/gamma activity and alpha-contaminated solid organic radioactive waste, and the pyrolysis of organic radioactive waste

Radioactive action code

International Nuclear Information System (INIS)

Anon.

1988-01-01

A new coding system, 'Hazrad', for buildings and transportation containers for alerting emergency services personnel to the presence of radioactive materials has been developed in the United Kingdom. The hazards of materials in the buildings or transport container, together with the recommended emergency action, are represented by a number of codes which are marked on the building or container and interpreted from a chart carried as a pocket-size guide. Buildings would be marked with the familiar yellow 'radioactive' trefoil, the written information 'Radioactive materials' and a list of isotopes. Under this the 'Hazrad' code would be written - three symbols to denote the relative radioactive risk (low, medium or high), the biological risk (also low, medium or high) and the third showing the type of radiation emitted, alpha, beta or gamma. The response cards indicate appropriate measures to take, eg for a high biological risk, Bio3, the wearing of a gas-tight protection suit is advised. The code and its uses are explained. (U.K.)

Intense ${^31-35}$Ar beams produced with a nanostructured CaO target at ISOLDE

CERN Document Server

Ramos, J P; Mendonça, T M; Seiffert, C; Senos, A M R; Fynbo, H O U; Tengblad, O; Briz, J A; Lund, M V; Koldste, G T; Carmona-Gallardo, M; Pesudo, V; Stora, T

2014-01-01

At the ISOLDE facility at CERN, thick targets are bombarded with highly energetic pulsed protons to produce radioactive ion beams (RIBs). The isotopes produced in the bulk of the material have to diffuse out of the grain and effuse throughout the porosity of the material to a transfer line which is connected to an ionizer, from which the charged isotopes are extracted and delivered for physics experiments. Calcium oxide (CaO) powder targets have been used to produce mainly neutron deficient argon and carbon RIBs over the past decades. Such targets presented unstable yields, either decaying over time or low from the beginning of operation. These problems were suspected to come from the degradation of the target microstructure (sintering due to high temperature and/or high proton intensity). In this work, a CaO microstructural study in terms of sintering was conducted on a nanostructured CaO powder synthesized from the respective carbonate. Taking the results of this study, several changes were made at ISOLDE i...

Isotope production potential at Sandia National Laboratories: Product, waste, packaging, and transportation

International Nuclear Information System (INIS)

Trennel, A.J.

1995-01-01

The U.S. Congress directed the U.S. Department of Energy to establish a domestic source of molybdenum-99, an essential isotope used in nuclear medicine and radiopharmacology. An Environmental Impact Statement for production of 99 Mo at one of four candidate sites is being prepared. As one of the candidate sites, Sandia National Laboratories is developing the Isotope Production Project. Using federally approved processes and procedures now owned by the U.S. Department of Energy, and existing facilities that would be modified to meet the production requirements, the Sandia National Laboratories' Isotope Project would manufacture up to 30 percent of the U.S. market, with the capacity to meet 100 percent of the domestic need if necessary. This paper provides a brief overview of the facility, equipment, and processes required to produce isotopes. Packaging and transportation issues affecting both product and waste are addressed, and the storage and disposal of the four low-level radioactive waste types generated by the production program are considered. Recommendations for future development are provided

Inelastic scattering of Ni and Zn isotopes off a proton target

Energy Technology Data Exchange (ETDEWEB)

Cortes Sua, Martha Liliana

2016-07-18

Inelastic proton scattering of {sup 70,72,74}Ni and {sup 76,78,80}Zn was performed at the RIBF facility of the RIKEN Nishina Center, Japan, as part of the first SEASTAR campaign. Radioactive isotopes were produced by the in-flight fission of a beam of {sup 238}U ions incident on a 3 mm thick Beryllium target. After production, neutron-rich radioactive isotopes were selected and identified on an event-by-event basis using the BigRIPS separator. Selected isotopes of interest were focused onto the liquid hydrogen target of the MINOS device and γ-rays from inelastic (p,p{sup '}) reactions were detected with the DALI2 array, consisting of 186 NaI crystals. Outgoing beam-like particles were identified using the ZeroDegree spectrometer. γ-rays produced in the reaction were Doppler corrected and the first 2{sup +} and 4{sup +} states in all the isotopes were identified. Detailed data analysis was performed including the implementation of algorithms that discriminate events where more than one particle was present. Using detailed Geant4 simulations, exclusive cross-sections for inelastic proton scattering were obtained. Deformation lengths were deduced from the experimental cross-sections using the coupled-channel calculation code ECIS-97. The deformations lengths of {sup 72,74}Ni and {sup 76,80}Zn were found to be fairly constant at a value of 0.8(2) fm, suggesting similar vibrational amplitudes, while the isomeric presence in the secondary beams of {sup 70}Ni and {sup 78}Zn allowed only lower limits for those two isotopes. By combining the deformation lengths with the known B(E2;0{sup +}{sub gs}→2{sup +}{sub 1}) values, the neutron-to-proton matrix element ratios, M{sub n}/M{sub p}, were obtained. A clear indication of the closed proton shell in the {sup 72,74}Ni could be observed, as M{sub n}/M{sub p}>N/Z, indicating an increased contribution of the neutrons to the vibrational amplitude. For the case of {sup 76,80}Zn, M{sub n}/M{sub p}

ISOGEN: Interactive isotope generation and depletion code

International Nuclear Information System (INIS)

Venkata Subbaiah, Kamatam

2016-01-01

ISOGEN is an interactive code for solving first order coupled linear differential equations with constant coefficients for a large number of isotopes, which are produced or depleted by the processes of radioactive decay or through neutron transmutation or fission. These coupled equations can be written in a matrix notation involving radioactive decay constants and transmutation coefficients, and the eigenvalues of thus formed matrix vary widely (several tens of orders), and hence no single method of solution is suitable for obtaining precise estimate of concentrations of isotopes. Therefore, different methods of solutions are followed, namely, matrix exponential method, Bateman series method, and Gauss-Seidel iteration method, as was followed in the ORIGEN-2 code. ISOGEN code is written in a modern computer language, VB.NET version 2013 for Windows operating system version 7, which enables one to provide many interactive features between the user and the program. The output results depend on the input neutron database employed and the time step involved in the calculations. The present program can display the information about the database files, and the user has to select one which suits the current need. The program prints the 'WARNING' information if the time step is too large, which is decided based on the built-in convergence criterion. Other salient interactive features provided are (i) inspection of input data that goes into calculation, (ii) viewing of radioactive decay sequence of isotopes (daughters, precursors, photons emitted) in a graphical format, (iii) solution of parent and daughter products by direct Bateman series solution method, (iv) quick input method and context sensitive prompts for guiding the novice user, (v) view of output tables for any parameter of interest, and (vi) output file can be read to generate new information and can be viewed or printed since the program stores basic nuclide concentration unlike other batch jobs. The sample

Computer study of isotope production for medical and industrial applications in high power accelerators

Science.gov (United States)

Mashnik, S. G.; Wilson, W. B.; Van Riper, K. A.

2001-07-01

Methods for radionuclide production calculation in a high power proton accelerator have been developed and applied to study production of 22 isotopes. These methods are readily applicable both to accelerator and reactor environments and to the production of other radioactive and stable isotopes. We have also developed methods for evaluating cross sections from a wide variety of sources into a single cross section set and have produced an evaluated library covering about a third of all natural elements that may be expanded to other reactions. A 684 page detailed report on this study, with 37 tables and 264 color figures, is available on the Web at http://t2.lanl.gov/publications/.

Separation efficiency of the MASHA facility for short-lived mercury isotopes

Science.gov (United States)

Rodin, A. M.; Belozerov, A. V.; Chernysheva, E. V.; Dmitriev, S. N.; Gulyaev, A. V.; Gulyaeva, A. V.; Itkis, M. G.; Kliman, J.; Kondratiev, N. A.; Krupa, L.; Novoselov, A. S.; Oganessian, Yu. Ts.; Podshibyakin, A. V.; Salamatin, V. S.; Siváček, I.; Stepantsov, S. V.; Vanin, D. V.; Vedeneev, V. Yu.; Yukhimchuk, S. A.; Granja, C.; Pospisil, S.

2014-06-01

The mass-separator MASHA built to identify Super Heavy Elements by their mass-to-charge ratios is described. The results of the off- and on-line measurements of its separation efficiency are presented. In the former case four calibrated leaks of noble gases were used. In the latter the efficiency was measured via 284 MeV Ar beam and with using the hot catcher. The ECR ion source was used in both cases. The -radioactive isotopes of mercury produced in the complete fusion reaction Ar+SmHg+xn were detected at the mass-separator focal plane. The half-lives and the separation efficiency for the short-lived mercury isotopes were measured. Potentialities of the MEDIPIX detector system have been demonstrated for future use at the mass-separator MASHA.

Climate and isotopic tracers

International Nuclear Information System (INIS)

Jean-Baptiste, Ph.

1997-01-01

The applications of natural radioactivity and isotopic measurements in the sciences concerning Earth and its atmosphere, are numerous: carbon 14 dating with the Tandetron apparatus at the Cea, measurement of oxygen 18 in coral or sediment limestone for the determination of ocean temperature and salinity, carbon 14 dating of corals for the determination of sea level variations, deuterium content in polar ice-cap leads to temperature variations determination; isotopic measurements also enable the determination of present climate features such as global warming, oceanic general circulation

Evaluation of {sup 18}F radioactive concentration in exhaust at cyclotron facility at Chosun University

Energy Technology Data Exchange (ETDEWEB)

Jeong, Cheol Ki; Jang, Han; Lee, Goung Jin [Dept. of Nuclear Engineering, Chsoun University, Gwangju (Korea, Republic of)

2016-11-15

the recent prevalence of PET examinations in Korea has led to an increase in the number of cyclotrons. the medical isotope 18F produced in most cyclotron facilities currently operating in Korea is emitted into the environment during the production of [{sup 18}F]FdG, a cancerdiagnosis reagent. the amount of [{sup 18}F]FdG synthesized determines the radioactive concentration of {sup 18}F in the exhaust. at some facilities, this amount temporarily exceeds the emission limit. In this study, we evaluated the {sup 18}F radioactivity concentration in the exhaust from the cyclotron facility at chosun university. the {sup 18}F radioactivity concentration was measured using an air sampler and a hPGe semiconductor detector. the measurements showed that the radioactive concentration of {sup 18}F in the exhaust at the cyclotron facility at Chosun university was the highest during [{sup 18}F]FdG synthesis but remained under the legal limit of 2,000 Bq m{sup -3}.

Isotope method for the recognition of groundwater formation in China's preselected high level radioactive waste disposal repository site

International Nuclear Information System (INIS)

Guo Yonghai; Wang Ju; Liu Shufen; Su Rui; Lu Chuanhe

2005-01-01

Yemaquan region in Beishan area. Gansu province, is one of the preselected sites of disposal repository for high level radioactive waste (HLW) in our country. Hydrogeological condition is an important aspect for site evaluation and the groundwater formation is a key factor to reflect the hydrogeological conditions for a certain area. Isotopic method is the one of the important means to determine the groundwater formation. Through the sampling and analysis of shallow groundwater isotopes of Yemaquan region, combined with geological, hydrogeological and hydrogeochemical characteristics, the issue of groundwater formation in the study region was discussed. The main cognition is that the groundwater in the region was formed from the infiltration of modern rainfall and the strong evaporation was happened for the shallow groundwater, which indicates the circulation conditions were relatively good for the shallow groundwater. This cognition provides very important hydrogeological information and basis for the evaluation of Yemaquan preselected site. (authors)

Radioactive ion beam production challenges at the Holifield Heavy Ion Research Facility

International Nuclear Information System (INIS)

Meigs, M.J.; Alton, G.D.; Dowling, D.T.; Haynes, D.L.; Jones, C.M.; Juras, R.C.; Lane, S.N.; Mills, G.D.; Mosko, S.W.; Olsen, D.K.; Tatum, B.A.

1992-01-01

The radioactive ion beam (RIB) project at the Holifield Heavy Ion Research Facility (HHIRF) will provide for reconfiguration of the HHIRF accelerator system to enable provision of low-intensity RIBs for nuclear and astrophysics research. As we have progressed with the design of the reconfiguration, we have encountered several challenges that were not immediately obvious when first contemplating the project. The challenges do not seem insurmountable but should keep life interesting for those of us doing the work. A brief review of the project will allow a better understanding of the challenges in RIB production. Radioactive ion beams will be produced with the Isotope Separator On-Line (ISOL) postacceleration technique. In particular, radioactive atoms will be produced by reactions in the thick stopping target of an ISOL-type target-ion source assembly using intense beams from the Oak Ridge Isochronous Cyclotron equipped with a light-ion internal source. This ISOL target-ion source assembly will be mounted on a high-voltage platform with a mass separator. The target ion source will operate at potentials up to 50 kV with respect to the high voltage platform. The radioactive atoms produced by nuclear reactions in the target diffuse to the surface of the heated target material, desorb from this surface, and effuse through a heated transfer tube into an ion source where ionization and extraction take place. Two types of ion sources will be initially considered. A Forced Electron Beam Induced Arc Discharge source, similar to those used by the ISOLDE facility at CERN and by the UNISOR facility at ORNL, will be built to produce positive ions. These positive ions will be focused through an alkali vapor charge-exchange canal to produce negative ions for tandem injection. In addition, a direct negative surface ionization addition or modification to the above source will be built and investigated

PRAMANA Cluster radioactivity in xenon isotopes

Indian Academy of Sciences (India)

exotic decay or cluster radioactivity was first predicted by sandulescu et al [1] in. 1980 on the basis of ... separator by 58Ni(58Ni, 2n) reaction and carbon clusters were searched for by means of solid state nuclear ..... Lett. 55, 582 (1985). [22] D N Poenaru, W Greiner, K Depta, M Ivascu, D Mazilu and A Sandulescu, At. Data.

Stable isotope deltas: Tiny, yet robust signatures in nature

Science.gov (United States)

Brand, Willi A.; Coplen, Tyler B.

2012-01-01

Although most of them are relatively small, stable isotope deltas of naturally occurring substances are robust and enable workers in anthropology, atmospheric sciences, biology, chemistry, environmental sciences, food and drug authentication, forensic science, geochemistry, geology, oceanography, and paleoclimatology to study a variety of topics. Two fundamental processes explain the stable isotope deltas measured in most terrestrial systems: isotopic fractionation and isotope mixing. Isotopic fractionation is the result of equilibrium or kinetic physicochemical processes that fractionate isotopes because of small differences in physical or chemical properties of molecular species having different isotopes. It is shown that the mixing of radioactive and stable isotope end members can be modelled to provide information on many natural processes, including 14C abundances in the modern atmosphere and the stable hydrogen and oxygen isotopic compositions of the oceans during glacial and interglacial times. The calculation of mixing fractions using isotope balance equations with isotope deltas can be substantially in error when substances with high concentrations of heavy isotopes (e.g. 13C, 2H, and 18O ) are mixed. In such cases, calculations using mole fractions are preferred as they produce accurate mixing fractions. Isotope deltas are dimensionless quantities. In the International System of Units (SI), these quantities have the unit 1 and the usual list of prefixes is not applicable. To overcome traditional limitations with expressing orders of magnitude differences in isotope deltas, we propose the term urey (symbol Ur), after Harold C. Urey, for the unit 1. In such a manner, an isotope delta value expressed traditionally as−25 per mil can be written as−25 mUr (or−2.5 cUr or−0.25 dUr; the use of any SI prefix is possible). Likewise, very small isotopic differences often expressed in per meg ‘units’ are easily included (e.g. either+0.015 ‰ or+15 per meg

Isotopes in action

International Nuclear Information System (INIS)

1987-01-01

For most people the obvious application of nuclear technology is in power generation. But there are many other uses for radioactive materials or for products made with their help. They are found in our factories, hospitals, offices and homes. ''Isotopes in Action'' looks at the many applications of radioisotopes in our society. (author)

Electric Dipole Moment Measurements with Rare Isotopes

International Nuclear Information System (INIS)

Chupp, Timothy

2016-01-01

The origin of matter is one of the deepest questions addressed by science and remains a mystery because our understanding of the Big Bang suggests that equal amounts of matter as antimatter would be created and annihilate leaving nothing from which stars, galaxies, planets and ultimately life as we know it was created. We know this is not the case in the universe, and so the explanation that the laws of physics can distinguish the difference of moving forward and backward in time and provide mechanisms that produce more matter that antimatter so that a little bit was left over. These same laws of physics affect our world today and would very slightly change the shape of an atom, stretching is along the direction of the spin of its nucleus. This subtle shape change has been searched in many systems - the neutron, atoms and molecules, but has not yet been detected, even as the motivation is strengthened by our understanding of their structure. We therefore look to new systems that have special features that make these effects stand out. Rare isotopes provide one possibility and specific radon atoms are our choice. We have developed techniques to make these measurements with short-lived radioactive atoms, studied the nuclei to provide deeper understanding of how these affect arise in such atoms (including radium) and developed new laser-based techniques to measure and control the magnetic fields necessary to perform these exquisitely sensitive measurements. In this work we have shown that radioactive radon atoms can be produced and transported to an apparatus that lines up the spins of the atoms. We have also shown that the nuclei of nearby radium are pear shaped and that the radon nuclei likely oscillate from one pear shape to its mirror reflection. We have also used the techniques which control nuclear spin to study the magnetic environment in a magnetically shielded room, which has the smallest magnetic field in a large volume in the universe. Measuring magnetic

Electric Dipole Moment Measurements with Rare Isotopes

Energy Technology Data Exchange (ETDEWEB)

Chupp, Timothy [Univ. of Michigan, Ann Arbor, MI (United States)

2016-11-11

The origin of matter is one of the deepest questions addressed by science and remains a mystery because our understanding of the Big Bang suggests that equal amounts of matter as antimatter would be created and annihilate leaving nothing from which stars, galaxies, planets and ultimately life as we know it was created. We know this is not the case in the universe, and so the explanation that the laws of physics can distinguish the difference of moving forward and backward in time and provide mechanisms that produce more matter that antimatter so that a little bit was left over. These same laws of physics affect our world today and would very slightly change the shape of an atom, stretching is along the direction of the spin of its nucleus. This subtle shape change has been searched in many systems - the neutron, atoms and molecules, but has not yet been detected, even as the motivation is strengthened by our understanding of their structure. We therefore look to new systems that have special features that make these effects stand out. Rare isotopes provide one possibility and specific radon atoms are our choice. We have developed techniques to make these measurements with short-lived radioactive atoms, studied the nuclei to provide deeper understanding of how these affect arise in such atoms (including radium) and developed new laser-based techniques to measure and control the magnetic fields necessary to perform these exquisitely sensitive measurements. In this work we have shown that radioactive radon atoms can be produced and transported to an apparatus that lines up the spins of the atoms. We have also shown that the nuclei of nearby radium are pear shaped and that the radon nuclei likely oscillate from one pear shape to its mirror reflection. We have also used the techniques which control nuclear spin to study the magnetic environment in a magnetically shielded room, which has the smallest magnetic field in a large volume in the universe. Measuring magnetic

Nuclide radioactive decay data uncertainties library

International Nuclear Information System (INIS)

Barabanova, D S; Zherdev, G M

2017-01-01

The results of the developing the library of uncertainties of radioactive decay data in the ABBN data library format are described. Different evaluations of uncertainties were compared and their effects on the results of calculations of residual energy release were determined using the test problems and experiment. Tables were generated in the ABBN format with the data obtained on the basis of libraries in ENDF-6 format. 3821 isotopes from the ENDF/B-7 data library, 3852 isotopes from the JEFF-3.11 data library and 1264 isotopes from the JENDL-4.0 data library were processed. It was revealed that the differences in the evaluations accepted in different decay data libraries are not so big, although they sometimes exceed the uncertainties assigned to the data in the ENDF/B-7 and JEFF-3.11 libraries, which as a rule, they agree with each other. On the basis of developed method it is supposed to create a library of data uncertainties for radioactive decay within the constant data system in FSUE RFNC-VNIIEF with its further connection with CRYSTAL module. (paper)

Laser spectroscopy of radioactive beams

International Nuclear Information System (INIS)

Otten, E.W.

1983-01-01

The problem of using the laser spectroscopy in investigations radioactive beams is considered. The main attention is payed to the isotope shift of nuclear charge radii delta 2 >. The general trend of delta 2 > is discussed. Predictions for delta>r 2 < in the framework of the droplet model are given. It is noted that two parameter interpretation of the isotope shift based on the droplet model works the better, the further the distance spans and the clearer the nuclear structure is

On models in the geochemistry of isotopes

International Nuclear Information System (INIS)

Wetzel, K.

1978-01-01

Models are playing an increasing role in the deepening of our understanding of the laws of occurrence of stable and radioactive isotopes in nature. The properties of concrete global and regional models of the geochemistry of isotopes are derived from a general model characterizing the cycling of chemical elements and their isotopes in nature. The importance of global models as well as the relationships between global and regional models are considered. The introduction of a parameter describing the velocity of both mass and isotope transfer, taking into consideration the global resources, renders possible the linkage of global models with regional ones. (author)

A combustion setup to precisely reference δ13C and δ2H isotope ratios of pure CH4 to produce isotope reference gases of δ13C-CH4 in synthetic air

Directory of Open Access Journals (Sweden)

H. Schaefer

2012-09-01

Full Text Available Isotope records of atmospheric CH4 can be used to infer changes in the biogeochemistry of CH4. One factor currently limiting the quantitative interpretation of such changes are uncertainties in the isotope measurements stemming from the lack of a unique isotope reference gas, certified for δ13C-CH4 or δ2H-CH4. We present a method to produce isotope reference gases for CH4 in synthetic air that are precisely anchored to the VPDB and VSMOW scales and have δ13C-CH4 values typical for the modern and glacial atmosphere. We quantitatively combusted two pure CH4 gases from fossil and biogenic sources and determined the δ13C and δ2H values of the produced CO2 and H2O relative to the VPDB and VSMOW scales within a very small analytical uncertainty of 0.04‰ and 0.7‰, respectively. We found isotope ratios of −39.56‰ and −56.37‰ for δ13C and −170.1‰ and −317.4‰ for δ2H in the fossil and biogenic CH4, respectively. We used both CH4 types as parental gases from which we mixed two filial CH4 gases. Their δ13C was determined to be −42.21‰ and −47.25‰ representing glacial and present atmospheric δ13C-CH4. The δ2H isotope ratios of the filial CH4 gases were found to be −193.1‰ and −237.1‰, respectively. Next, we mixed aliquots of the filial CH4 gases with ultrapure N2/O2 (CH4 ≤ 2 ppb producing two isotope reference gases of synthetic air with CH4 mixing ratios near atmospheric values. We show that our method is reproducible and does not introduce isotopic fractionation for δ13C within the uncertainties of our detection limit (we cannot conclude this for δ2H because our system is currently not prepared for δ2H-CH4 measurements in air samples. The general principle of our method can be applied to produce synthetic isotope reference gases targeting δ2H-CH4 or other gas species.

Use of environmental isotope techniques in groundwater hydrology

International Nuclear Information System (INIS)

Tirumalesh, K.; Shivanna, K.

2009-01-01

Environmental isotopes (stable and radioactive) have been used as tracers for investigating various hydrological problems. Wide variation in isotopic distribution ( 2 H, 13 C, 18 O, 15 N, 35 S, 3 H and 14 C) in the environment help in identifying the source, origin, pathways and processes affecting the system under consideration. In this article, a few Indian case studies covering some of the very important isotope applications in groundwater hydrology are briefly summarized. (author)

Medical Isotope Production Analyses In KIPT Neutron Source Facility

International Nuclear Information System (INIS)

Talamo, Alberto; Gohar, Yousry

2016-01-01

Medical isotope production analyses in Kharkov Institute of Physics and Technology (KIPT) neutron source facility were performed to include the details of the irradiation cassette and the self-shielding effect. An updated detailed model of the facility was used for the analyses. The facility consists of an accelerator-driven system (ADS), which has a subcritical assembly using low-enriched uranium fuel elements with a beryllium-graphite reflector. The beryllium assemblies of the reflector have the same outer geometry as the fuel elements, which permits loading the subcritical assembly with different number of fuel elements without impacting the reflector performance. The subcritical assembly is driven by an external neutron source generated from the interaction of 100-kW electron beam with a tungsten target. The facility construction was completed at the end of 2015, and it is planned to start the operation during the year of 2016. It is the first ADS in the world, which has a coolant system for removing the generated fission power. Argonne National Laboratory has developed the design concept and performed extensive design analyses for the facility including its utilization for the production of different radioactive medical isotopes. 99 Mo is the parent isotope of 99m Tc, which is the most commonly used medical radioactive isotope. Detailed analyses were performed to define the optimal sample irradiation location and the generated activity, for several radioactive medical isotopes, as a function of the irradiation time.

Medical Isotope Production Analyses In KIPT Neutron Source Facility

Energy Technology Data Exchange (ETDEWEB)

Talamo, Alberto [Argonne National Lab. (ANL), Argonne, IL (United States); Gohar, Yousry [Argonne National Lab. (ANL), Argonne, IL (United States)

2016-01-01

Medical isotope production analyses in Kharkov Institute of Physics and Technology (KIPT) neutron source facility were performed to include the details of the irradiation cassette and the self-shielding effect. An updated detailed model of the facility was used for the analyses. The facility consists of an accelerator-driven system (ADS), which has a subcritical assembly using low-enriched uranium fuel elements with a beryllium-graphite reflector. The beryllium assemblies of the reflector have the same outer geometry as the fuel elements, which permits loading the subcritical assembly with different number of fuel elements without impacting the reflector performance. The subcritical assembly is driven by an external neutron source generated from the interaction of 100-kW electron beam with a tungsten target. The facility construction was completed at the end of 2015, and it is planned to start the operation during the year of 2016. It is the first ADS in the world, which has a coolant system for removing the generated fission power. Argonne National Laboratory has developed the design concept and performed extensive design analyses for the facility including its utilization for the production of different radioactive medical isotopes. ⁹⁹Mo is the parent isotope of ^99mTc, which is the most commonly used medical radioactive isotope. Detailed analyses were performed to define the optimal sample irradiation location and the generated activity, for several radioactive medical isotopes, as a function of the irradiation time.

Distribution of isotopes produced in superconductor YBa2Cu3O7-x and ferroelectric PbZr0.54Ti0.46O3 under irradiation by high-energy charged particles

International Nuclear Information System (INIS)

Didik, V.A.; Malkovich, R.Sh.; Skoryatina, E.A.; Kozlovskij, V.V.

1998-01-01

The concentration profiles of transmutation radioactive isotopes, formed in the YBa 2 Cu 3 O 7-x superconductor and PbZr 0.54 Ti 0.46 O 3 ferroelectric under high-energy proton radiation (with 10 and 15 MeV energy), deuterons (4 MeV), the 3 He and 4 He nuclei (20 MeV), are studied. Two types of the concentration profiles: monotonous ones and profiles with the maximum are identified. It is shown that the isotope profile is determined by the character of energy dependence of the nuclear reaction cross section, leading to formation of the given isotope

Fred Hoyle, primary nucleosynthesis and radioactivity

Science.gov (United States)

Clayton, Donald D.

2008-10-01

Primary nucleosynthesis is defined as that which occurs efficiently in stars born of only H and He. It is responsible not only for increasing the metallicity of the galaxy but also for the most abundant gamma-ray-line emitters. Astrophysicists have inappropriately cited early work in this regard. The heavily cited B2FH paper (Burbidge et al., 1957) did not effectively address primary nucleosynthesis whereas Hoyle (Hoyle, 1954) had done so quite thoroughly in his infrequently cited 1954 paper. Even B2FH with Hoyle as coauthor seems strangely to not have appreciated what Hoyle (Hoyle, 1954) had achieved. I speculate that Hoyle must not have thoroughly proofread the draft written in 1956 by E.M. and G.R. Burbidge. The clear roadmap of primary nucleosynthesis advanced in 1954 by Hoyle describes the synthesis yielding the most abundant of the radioactive isotopes for astronomy, although that aspect was unrealized at the time. Secondary nucleosynthesis has also produced many observable radioactive nuclei, including the first gamma-ray-line emitter to be discovered in the galaxy and several others within stardust grains. Primary gamma-ray emitters would have been even more detectable in the early galaxy, when the birth rate of massive stars was greater; but secondary emitters, such as 26Al, would have been produced with smaller yield then owing to smaller abundance of seed nuclei from which to create them.

Management of Radioactive Wastes

International Nuclear Information System (INIS)

Tchokosa, P.

2010-01-01

Management of Radioactive Wastes is to protect workers and the public from the radiological risk associated with radioactive waste for the present and future. It application of the principles to the management of waste generated in a radioisotope uses in the industry. Any material that contains or is contaminated with radionuclides at concentrations or radioactivity levels greater than ‘exempt quantities’ established by the competent regulatory authorities and for which no further use is foreseen or intended. Origin of the Radioactive Waste includes Uranium and Thorium mining and milling, nuclear fuel cycle operations, Operation of Nuclear power station, Decontamination and decommissioning of nuclear facilities and Institutional uses of isotopes. There are types of radioactive waste: Low-level Waste (LLW) and High-level Waste. The Management Options for Radioactive Waste Depends on Form, Activity, Concentration and half-lives of the radioactive waste, Storage and disposal methods will vary according to the following; the radionuclides present, and their concentration, and radio toxicity. The contamination results basically from: Contact between radioactive materials and any surface especially during handling. And it may occur in the solid, liquid or gas state. Decontamination is any process that will either reduce or completely remove the amount of radionuclides from a contaminated surface

Mass measurements on radioactive isotopes using the ISOLTRAP spectrometer

CERN Document Server

Dilling, J; Kluge, H J; Kohl, A; Lamour, E; Marx, G; Schwarz, S C; Bollen, G; Kellerbauer, A G; Moore, R B; Henry, S

2000-01-01

ISOLTRAP is a Penning trap mass spectrometer installed at the on line isotope separator ISOLDE at CERN. Direct measurements of the masses of short lived radio isotopes are performed using the existing triple trap system. This consists of three electromagnetic traps in tandem: a Paul trap to accumulate and bunch the 60 keV dc beam, a Penning trap for cooling and isobar separation, and a precision Penning trap for the determination of the masses by cyclotron resonance. Measurements of masses of unknown mercury isotopes and in the vicinity of doubly magic /sup 208/Pb are presented, all with an accuracy of delta m/m approximately=1*10/sup -7/. Developments to replace the Paul trap by a radiofrequency quadrupole ion guide system to increase the collection efficiency are presently under way and the status is presented. (10 refs).

Current status of radio-isotopes utilization

Energy Technology Data Exchange (ETDEWEB)

Singh, M [Banaras Hindu Univ. (India)

1974-08-01

Utilization of radioisotopes were reviewed briefly in a categorized manner. In plant biochemistry, long lived radioactive carbon ,/sup 14/C, was applied to clarify such metabolic processes as photosynthesis, respiration and protein synthesis, etc., while radioactive oxygen ,/sup 18/O, was used to study the O/sub 2/ generation mechanism. Radioactive phosphorus ,/sup 32/P, was used to detect the amount, grain size of phosphatic fertilizer as well as the time and depth for better utilization. Radioactive sulphur ,/sup 35/S, and nitrogen ,/sup 15/N, could be of use in studies of protein metabolism in plants. Radioactive tracers of other minerals such as N, P, K, Ca, Mg, Zn, Mo, B, and Co were also used to detect their specific role in plants. Use of radioactive isotopes in protein synthesis and transfer of genetic information was described. Radioactive iodine ,/sup 131/I, binding capacity of milk proteins, and radio trace studies in the iodine turn over in the use of radioactive iodine were summarized.

Materials science and biophysics applications at the ISOLDE radioactive ion beam facility

Energy Technology Data Exchange (ETDEWEB)

Wahl, U., E-mail: uwahl@itn.pt [Instituto Tecnologico e Nuclear, Estrada Nacional 10, 2686-953 Sacavem (Portugal); Centro de Fisica Nuclear da Universidade de Lisboa, Av. Prof. Gama Pinto 2, 1649-003 Lisboa (Portugal)

2011-12-15

The ISOLDE isotope separator facility at CERN provides a variety of radioactive ion beams, currently more than 800 different isotopes from {approx}70 chemical elements. The radioisotopes are produced on-line by nuclear reactions from a 1.4 GeV proton beam with various types of targets, outdiffusion of the reaction products and, if possible, chemically selective ionisation, followed by 60 kV acceleration and mass separation. While ISOLDE is mainly used for nuclear and atomic physics studies, applications in materials science and biophysics account for a significant part (currently {approx}15%) of the delivered beam time, requested by 18 different experiments. The ISOLDE materials science and biophysics community currently consists of {approx}80 scientists from more than 40 participating institutes and 21 countries. In the field of materials science, investigations focus on the study of semiconductors and oxides, with the recent additions of nanoparticles and metals, while the biophysics studies address the toxicity of metal ions in biological systems. The characterisation methods used are typical radioactive probe techniques such as Moessbauer spectroscopy, perturbed angular correlation, emission channeling, and tracer diffusion studies. In addition to these 'classic' methods of nuclear solid state physics, also standard semiconductor analysis techniques such as photoluminescence or deep level transient spectroscopy profit from the application of radioactive isotopes, which helps them to overcome their chemical 'blindness' since the nuclear half life of radioisotopes provides a signal that changes in time with characteristic exponential decay or saturation curves. In this presentation an overview will be given on the recent research activities in materials science and biophysics at ISOLDE, presenting some of the highlights during the last five years, together with a short outlook on the new developments under way.

Radioactive contamination of the environmental samples in Hanoi in 1989

International Nuclear Information System (INIS)

Dang Huy Uyen; Bui Van Loat; Dang Phuong Nam; Cao Anh Duc; Pham Quang Dien; Nguyen Hao Quang

1990-01-01

More than 30 environmental samples from soil, paddy, rice, fruits, vegetables and beans, sesame, tea, bananas, fishes at Hanoi markets in 1989 were analysed by gamma ray spectrometry with the low background system for studying natural and artificial radioactive elements. Among several samples from Hanoi in such kind as cultivated soils, tea, dried bamboo shoots, isotope Cs 137 that used be generated from nuclear explosives was found with contents (30 - 1000) x 10 -5 Bq/g; Cs 137 contents in Japanese rice (0.4 - 3) x 10 -5 Bq/g. Cs 137 is radioactive so Cs 137 contents in Vietnamese rice are 300 times higher than Cs 137 contents in Japanese rice but they are hundred times lower than international standard. Among vegetables, fruits, shrimps, fishes in Hanoi markets, artificial isotopes were not found and natural isotopes were few. Even radioactive daughter and granddaughter in uranium series in potatoes were not found. In some samples K 40 was also appeared, for example in cultivated soils (0.78 Bq/g), in dried bamboo shoots (0.73 Bq/g). (author). 2 refs., 3 figs

$\\beta$-delayed fission, laser spectroscopy and shape-coexistence studies with radioactive At beams

CERN Multimedia

We propose to study the $\\beta$-delayed fission, laser spectroscopy and radioactive decay of the newly available pure beams of neutron-deficient and neutron-rich astatine (Z=85) isotopes. The fission probability and the fission fragment distribution of the even-even isotopes $^{194,196}$Po following the $\\beta$-decay of the isotopes $^{194,196}$At will be studied with the Windmill setup. In-source laser spectroscopy will be performed on the entire astatine isotopic chain, using a combination of the Windmill setup, ISOLTRAP MR-ToF and ISOLDE Faraday. Radioactive decay data will be acquired at the Windmill setup throughout those studies and contribute to the global understanding of the phenomenon of shape coexistence in the neutron-deficient lead region.

Production of radioactive nuclides in inverse reaction kinematics

International Nuclear Information System (INIS)

Traykov, E.; Rogachevskiy, A.; Bosswell, M.; Dammalapati, U.; Dendooven, P.; Dermois, O.C.; Jungmann, K.; Onderwater, C.J.G.; Sohani, M.; Willmann, L.; Wilschut, H.W.; Young, A.R.

2007-01-01

Efficient production of short-lived radioactive isotopes in inverse reaction kinematics is an important technique for various applications. It is particularly relevant when the isotope of interest is only a few nucleons away from a stable isotope. In this article production via charge exchange and stripping reactions in combination with a magnetic separator is explored. The relation between the separator transmission efficiency, the production yield, and the choice of beam energy is discussed. The results of some exploratory experiments will be presented

Theoretical study on production of heavy neutron-rich isotopes around the N=126 shell closure in radioactive beam induced transfer reactions

Directory of Open Access Journals (Sweden)

Long Zhu

2017-04-01

Full Text Available In order to produce more unknown neutron-rich nuclei around N=126, the transfer reactions 136Xe + 198Pt, 136–144Xe + 208Pb, and 132Sn + 208Pb are investigated within the framework of the dinuclear system (DNS model. The influence of neutron excess of projectile on production cross sections of target-like products is studied through the reactions 136,144Xe + 208Pb. We find that the radioactive projectile 144Xe with much larger neutron excess is favorable to produce neutron-rich nuclei with charge number less than the target rather than produce transtarget nuclei. The incident energy dependence of yield distributions of fragments in the reaction 132Sn + 208Pb are also studied. The production cross sections of neutron-rich nuclei with Z=72–77 are predicted in the reactions 136–144Xe + 208Pb and 132Sn + 208Pb. It is noticed that the production cross sections of unknown neutron-rich nuclei in the reaction 144Xe + 208Pb are at least two orders of magnitude larger than those in the reaction 136Xe + 208Pb. The radioactive beam induced transfer reactions 139,144Xe + 208Pb, considering beam intensities proposed in SPIRAL2 (Production System of Radioactive Ion and Acceleration On-Line project as well, for production of neutron-rich nuclei around the N=126 shell closure are investigated for the first time. It is found that, in comparison to the stable beam 136Xe, the radioactive beam 144Xe shows great advantages for producing neutron-rich nuclei with N=126 and the advantages get more obvious for producing nuclei with less charge number.

Helium isotopes in rocks, waters and gases of the earth's crust

International Nuclear Information System (INIS)

Tolstikhin, L.H.

1984-01-01

In this chapter the distribution of helium isotopes in various samples (rocks, minerals, terrestrial fluids, gases etc.) is interpreted from the genetic point of view, namely what sources and processes provide the abundance of helium isotopes observed in a sample. The mixing of mantle, juvenile helium with pure radiogenic helium is the main process responsible for the helium isotope composition in any sample of the earth's crust, the share of each component (reflected in the 3 He/ 4 He ratio) depending on the history of the tectono-magnetic activity in the given region. A specific chemical composition of a rock or mineral, peculiarities of losses or trapping and a peculiar kind of distribution of radioactive elements can lead to unusual isotopic ratios of 3 He/ 4 He in radiogenic helium. Lastly, technogenic radioactive isotopes are widespread in nature; one of them, tritium ( 3 H), yields 3 He excess in terrestrial waters. (orig.)

Chemistry, spectroscopy and isotope separation of zirconium and its compounds as revealed by laser diagnostics of laser produced metal beams

International Nuclear Information System (INIS)

Hackett, P.A.; Humphries, M.; Rayner, D.M.; Bourne, O.L.; Mitchell, A.

1986-01-01

Recent work from the author's laboratory on zirconium beams is reviewed. Zirconium metal beams have been produced by laser vaporization of solid zirconium targets coupled with supersonic expansion of helium gas. The resultant supersonic metal beam is shown to present an ideal environment for various spectroscopic techniques. The state distribution of zirconium atoms in the beam is obtained from low resolution laser induced fluorescence (LIF) studies. High resolution LIF studies give information on the hyperfine splitting in the ground state of the zirconium-91 isotope. Information on the hyperfine splitting in the excited state is obtained from quantum beat spectroscopy. Low resolution 2 color multiphoton ionization spectroscopy using a XeCl laser allows isotope separation of all isotopes of zirconium. These metal beams are highly reactive and can be used to produce novel chemical species. The results of two studies in which a reactant is added to the expansion gas are reported here. Zirconium oxide (ZrO), a molecule observed in the emission spectra of cool stars and in laboratory studies at high temperatures, is produced in a low temperature, collision free environment by adding small quantities of oxygen to the expansion gas. Zirconium fluoride (ZrF), a molecule previously unobserved, is produced by the addition of small quantities of CF/sub 4/

Laboratory study of the radioactivity from fission products in microscopic fallout particles

International Nuclear Information System (INIS)

Smith, H.A.; Ward, T.E.; Wesick, J.

1978-01-01

An experiment is described wherein simple γ-ray detection and analysis techniques were utilized to study the radioactivity in local precipitation. Gamma spectra from filtered particulate, evaporation residue, and water from a sample of freshly fallen snow were counted, and the relative amount of several radionuclides present were identified. These data show that several isotopes produced in the recent Chinese nuclear detonation (Lop Nor testing ground, Sinkiang Province, 17 November 1976) are observable. Furthermore the data are sufficient to estimate the date of the detonation and to determine some of the characteristics of the explosion

Stable isotopes

International Nuclear Information System (INIS)

Evans, D.K.

1986-01-01

Seventy-five percent of the world's stable isotope supply comes from one producer, Oak Ridge Nuclear Laboratory (ORNL) in the US. Canadian concern is that foreign needs will be met only after domestic needs, thus creating a shortage of stable isotopes in Canada. This article describes the present situation in Canada (availability and cost) of stable isotopes, the isotope enrichment techniques, and related research programs at Chalk River Nuclear Laboratories (CRNL)

p-process xenon isotope anomalies in stardust grains from meteorites

International Nuclear Information System (INIS)

Ott, U.

2013-01-01

Full text: In measurements on 'bulk' samples of meteorites isotopic variations due to the p-process usually have taken a backseat compared to such in s- or r-isotopes, and, in the best case, can be qualitatively attributed to the p-process, with little to no inferences concerning detailed isotopic yields. The situation is different for grains of stardust that survived in primitive meteorites. In fact, isotopically strange xenon was the key feature that led to the first identification of a stardust mineral, nanodiamonds containing xenon with overabundances of up to a factor of ∼2 in both the r-only (≡H-Xe) and p-only (≡L-Xe) isotopes. Relative excesses of the two r-only isotopes ( 134 Xe, 136 Xe) as well as of the two p-only isotopes ( 124 Xe, 126 Xe) are not equal, hence the processes responsible for HL-xenon must differ from the 'average' r- and p-processes as reflected in solar system abundances. However, while considerable effort has been put into explaining H-Xe, there has been little work on the p-side (L-Xe). Relying on scarce nuclear data, Heymann and Dziczkaniec have studied photodisintegration reactions of Xe and Ba seeds in intermediate zones of supernovae and found that the relative production of the p-Xe isotopes depends sensitively on the yield of the (γ, α) reaction on 128 Ba. Another suggestion - applicable to both the r- and p-anomalies in diamond xenon - is that of a 'rapid separation' between stable Xe isotopes and radioactive precursors produced in the 'standard' p- (as well as r-) process. For the p-isotopes to work, this would require the bulk (87%) of 126 Xe to be produced via the 126 Ba precursor, with a half live of ∼100 minutes, in order to explain the high 124 Xe/ 126 Xe. In contrast to diamond xenon, xenon in silicon carbide contains - besides the component from the s-process in their parent AGB stars - 'almost normal' Xe, with indications for 124 Xe/ 126 Xe being few (∼8)% lower than in solar Xe.

Chernobyl radioactivity in grain produced in Greece in 1986

International Nuclear Information System (INIS)

Dominici, G.; Malvicini, A.; Panetsos, F.

1988-01-01

The Chernobyl radioactive cloud reached Greece in the first days of May 1986. During this period, the gain was in maximum growth; therefore, in absorbing the radionuclides it has become an excellent indicator of the deposited radioactivity. Measurements carried out in grain samples which were obtained from Greece are reported and some conclusions regarding population doses are presented

Radioactivity and tobacco; Radioactivite et tabac

Energy Technology Data Exchange (ETDEWEB)

Nifenecker, H. [Centre National de la Recherche Scientifique (IN2P3/CNRS), 38 - Grenoble (France)

2006-07-01

We drew the parallel between the effects on the health, in particular carcinogenic, of irradiation and tobacco. As regards this last one the carcinogenic main part of its activity is, doubtless, of chemical origin (tars and nicotine), but a part could be due to the radioactivity. Indeed, the tobacco possesses an activity due to isotopes {sup 210}Pb and {sup 210}Po, daughter products of radon. This activity is 10 pico-becquerel by package of cigarette. The radioactive isotopes settle on the lung mucous membrane. The Academy of Sciences (US) so estimates the annual dose delivered in lungs to approximately 80 milli-sievert. This relatively important dose is however delivered only in a small fraction of the lung tissue (approximately 250 cm{sup 3}). Of this fact it contributes only weakly to the carcinogenic effect of the tobacco. (N.C.)

Radioactive waste management information, 1982 summary and record-to-date

International Nuclear Information System (INIS)

Cassidy, G.B.

1983-07-01

This document summarizes radioactive waste data records for the Idaho National Engineering Laboratory (INEL) compiled since 1952. Kinds of information include volume, radioactivity, isotopic identity, origin, and decay status. The radioactive waste data presented was obtained from the INEL Radioactive Waste Management Information System (RWMIS). This report is updated annually to incorporate waste management data for the current year and reflects changes in previous annual reports. Changes are made to more accurately reflect the current status of waste operations at the INEL

Custom synthesis of isotope-labelled Apis mellifera Pheromone

International Nuclear Information System (INIS)

Conanan, Aida P.; Cortes, Nicole Marie A.; Daguno, Cristel Lyn R.; Templonuevo, Jose Angelo A.; Sucgang, Raymond J.

2012-01-01

The object of this study is to determine the optimum conditions for the synthesis of the isotope-labelled isopentyl acetate. Isopentyl acetate is widely used as a raw material in industries, in syntheses, and is utilized as a sex attractant (pheromone) by the bee species, Apis mellifera. The isotope labelling of isopentyl acetate will allow tracking of the fate and movement of the isopentyl acetate in the environment, in chemical transformations, and in biological systems. Esterification by alcoholysis of acetic acid was optimized for the preparation of Carbon-14( 14 C)-labelled isopentyl acetate from 14 C-labelled acetic acid and isoamyl alcohol. The different conditions studied were: (1) The effects of acid catalysis and/or reflux on the incorporation and retention of the isotope label on the product. The efficiency of label incorporation and retention was determined through the beta radioactivity of Carbon 14 in each of the synthetic constructs. Determination of the beta radioactivity concentration of 14 C in the isopentyl acetate product was done using low level liquid scintillation spectrometry. Each of the synthetic products was mixed with Ultima Gold scintillation cocktail in a low potassium glass scintillation vial, and analysed in a low-level Wallac 1414 scintillation counter. The application of catalysis without reflux resulted in the highest yield (35%). The same condition also resulted in the highest abundance of carbon isotope label with 2.40 Bequerels per cubic centimetre, Bq/cc (measurement unit for radioactivity). (author)

Technology developments for the identification, mapping, characterisation and segregation of radioactive contamination

International Nuclear Information System (INIS)

Smith, R.; Beddow, H.; Adsley, T.; Pearman, I.; Sweeney, A.; Smith, W.; Blythe, M.; Davies, M.

2015-01-01

The history of activities in the UK dealing with radioactive materials has led to many sites being contaminated by various radioactive isotopes. These come from a number of industries and educational activities such as nuclear power development, luminising works, research facilities and the oil and gas industry. These isotopes include radium, lead, polonium, thorium, uranium and trans-uranic elements. To remediate these sites it is essential that the isotopes are identified and quantified to enable the appropriate strategy to be developed and the most cost-efficient decontamination or sorting processes to be implemented. Nuvia has developed and implemented a suite of technologies to map the location of and to recover and process radioactive materials during remedial operations. These have been developed over a number of years to meet the requirements for both an effective remediation operation and to comply with the relevant regulatory requirements. This paper will describe these developments and give examples of their deployment in a diverse range of situations.(authors)

Application of carbon isotopes to detect seepage out of coalbed natural gas produced water impoundments

International Nuclear Information System (INIS)

Sharma, Shikha; Baggett, Joshua K.

2011-01-01

Highlights: → Coalbed natural gas extraction results in large amount of produced water. → Risk of deterioration of ambient water quality. → Carbon isotope natural tracer for detecting seepage from produced water impoundments. - Abstract: Coalbed natural gas (CBNG) production from coal bed aquifers requires large volumes of produced water to be pumped from the subsurface. The produced water ranges from high quality that meets state and federal drinking water standards to low quality due to increased salinity and/or sodicity. The Powder River Basin of northeastern Wyoming is a major coalbed natural gas producing region, where water quality generally decreases moving from the southeastern portion of the basin towards the center. Most produced water in Wyoming is disposed into impoundments and other surface drainages, where it may infiltrate into shallow groundwater. Groundwater degradation caused by infiltration of CBNG produced water holding impoundments into arid, soluble salt-rich soils is an issue of immense importance because groundwater is a major source for stock water, irrigation, and drinking water for many small communities in these areas. This study examines the potential of using stable C isotope signatures of dissolved inorganic C (δ 13 C DIC ) to track the fate of CBNG produced water after it is discharged into the impoundments. Other geochemical proxies like the major cations and major anions were used in conjunction with field water quality measurements to understand the geochemical differences between CBNG produced waters and ambient waters in the study area. Samples were collected from the CBNG discharge outfalls, produced water holding impoundments, and monitoring wells from different parts of the Powder River Basin and analyzed for δ 13 C DIC . The CBNG produced waters from outfalls and impoundments have positive δ 13 C DIC values that fall within the range of +12 per mille to +22 per mille, distinct from the ambient regional surface and

Isotope hydrology and its impact in the developing world

International Nuclear Information System (INIS)

Verhagen, B.Th.

2003-01-01

Ground water has increasingly taken its place in the provision of safe, potable supply in the developing world. Large investments have been made in infrastructural development for rural ground water supply schemes, but far too little attention has been given to assess the sustainability of these supplies. Overexploitation of aquifers, evident in failing boreholes and deteriorating water quality, has become a world-wide concern. Developments in physics half a century ago established the basis of isotope hydrology. Radioactive isotopes give information on ground water dynamics and recharge rates whilst non-radioactive - or stable - isotopes indicate origins of ground water and delineate ground water bodies. Environmental isotope hydrology is increasingly seen as a powerful discipline in assessing ground water systems. This is particularly important in developing environments, where historical data is rarely available. Brief examples are presented of isotope applications to collaborative ground water studies conducted at the University of the Witwatersrand. Recharge estimates based on isotope 'snapshot' data conform well with results from subsequent long-term water level observations in the Kalahari of Botswana. The importance is demonstrated of irrigation return flow and pollution hazard to the Lomagundi dolomite of Zimbabwe. Isotopes suggest the source of high nitrate concentrations to an important ground water supply in Tanzania. Mechanisms of the release of arsenic into millions of tube wells in Bangladesh are put into perspective. Isotope hydrology as appropriate technology is highlighted in terms of its cost-effectiveness and the investigative empowerment of local investigators. (author)

Naturally Occurring Radioactive Materials (NORM)

International Nuclear Information System (INIS)

Gray, P.

1997-01-01

This paper discusses the broad problems presented by Naturally Occuring Radioactive Materials (NORM). Technologically Enhanced naturally occuring radioactive material includes any radionuclides whose physical, chemical, radiological properties or radionuclide concentration have been altered from their natural state. With regard to NORM in particular, radioactive contamination is radioactive material in an undesired location. This is a concern in a range of industries: petroleum; uranium mining; phosphorus and phosphates; fertilizers; fossil fuels; forestry products; water treatment; metal mining and processing; geothermal energy. The author discusses in more detail the problem in the petroleum industry, including the isotopes of concern, the hazards they present, the contamination which they cause, ways to dispose of contaminated materials, and regulatory issues. He points out there are three key programs to reduce legal exposure and problems due to these contaminants: waste minimization; NORM assesment (surveys); NORM compliance (training)

Naturally Occurring Radioactive Materials (NORM)

Energy Technology Data Exchange (ETDEWEB)

Gray, P. [ed.

1997-02-01

This paper discusses the broad problems presented by Naturally Occuring Radioactive Materials (NORM). Technologically Enhanced naturally occuring radioactive material includes any radionuclides whose physical, chemical, radiological properties or radionuclide concentration have been altered from their natural state. With regard to NORM in particular, radioactive contamination is radioactive material in an undesired location. This is a concern in a range of industries: petroleum; uranium mining; phosphorus and phosphates; fertilizers; fossil fuels; forestry products; water treatment; metal mining and processing; geothermal energy. The author discusses in more detail the problem in the petroleum industry, including the isotopes of concern, the hazards they present, the contamination which they cause, ways to dispose of contaminated materials, and regulatory issues. He points out there are three key programs to reduce legal exposure and problems due to these contaminants: waste minimization; NORM assesment (surveys); NORM compliance (training).

Process for producing zeolite adsorbent and process for treating radioactive liquid waste with the zeolite adsorbent

International Nuclear Information System (INIS)

Motojima, K.; Kawamura, F.

1984-01-01

Zeolite is contacted with an aqueous solution containing at least one of copper, nickel, cobalt, manganese and zinc salts, preferably copper and nickel salts, particularly preferably copper salt, in such a form as sulfate, nitrate, or chloride, thereby adsorbing the metal on the zeolite in its pores by ion exchange, then the zeolite is treated with a water-soluble ferrocyanide compound, for example, potassium ferrocyanide, thereby forming metal ferrocyanide on the zeolite in its pores. Then, the zeolite is subjected to ageing treatment, thereby producing a zeolite adsorbent impregnated with metal ferrocyanide in the pores of zeolite. The adsorbent can selectively recover cesium with a high percent cesium removal from a radioactive liquid waste containing at least radioactive cesium, for example, a radioactive liquid waste containing cesium and such coexisting ions as sodium, magnesium, calcium and carbonate ions at the same time at a high concentration. The zeolite adsorbent has a stable adsorbability for a prolonged time

Radiological quality of packaged waters produced in France

International Nuclear Information System (INIS)

Franques, Nathalie; Perrin, Marie-Line; Godet, Jean-Luc; Pineau, Cyril; Loyen, Jeanne; Brassac, Annette; Gleizes, Marc; Baudry, Michel

2013-09-01

Based on radionuclide and uranium analyses performed in 2012 by the IRSN on packaged waters produced in France, this report presents the main results on this national survey. The objectives were a systematic measurement of radioactivity indicators, a systematic measurement of uranium content, and a limited measurement of radon-222 content in some samples. After some recalls on the notions of radioactivity and exposure, on uranium and radon properties, and of the present regulation, this report presents the adopted methodology, and discusses the range and limitation of this study. It presents and comments the results of systematic analyses of spring and natural mineral waters (presence of tritium, global beta and alpha activity, uranium concentration), the results of measurements of radon-222, and the results of additional analyses of spring and natural mineral waters (main radionuclides, radium-226, uranium isotopes, other radionuclides). It reports the calculation of doses and the interpretation of results for waters which have been submitted to additional analyses

Radioactive and stable cesium isotope distributions and dynamics in Japanese cedar forests.

Science.gov (United States)

Yoschenko, Vasyl; Takase, Tsugiko; Hinton, Thomas G; Nanba, Kenji; Onda, Yuichi; Konoplev, Alexei; Goto, Azusa; Yokoyama, Aya; Keitoku, Koji

2018-06-01

Dynamics of the Fukushima-derived radiocesium and distribution of the natural stable isotope 133 Cs in Japanese cedar (Cryptomeria japonica D. Don) forest ecosystems were studied during 2014-2016. For the experimental site in Yamakiya, Fukushima Prefecture, we present the redistribution of radiocesium among ecosystem compartments during the entire observation period, while the results obtained at another two experimental site were used to demonstrate similarity of the main trends in the Japanese forest ecosystems. Our observations at the Yamakiya site revealed significant redistribution of radiocesium between the ecosystem compartments during 2014-2016. During this same period radionuclide inventories in the aboveground tree biomass were relatively stable, however, radiocesium in forest litter decreased from 20 ± 11% of the total deposition in 2014 to 4.6 ± 2.7% in 2016. Radiocesium in the soil profile accumulated in the 5-cm topsoil layers. In 2016, more than 80% of the total radionuclide deposition in the ecosystem resided in the 5-cm topsoil layer. The radiocesium distribution between the aboveground biomass compartments at Yamakiya during 2014-2016 was gradually approaching a quasi-equilibrium distribution with stable cesium. Strong correlations of radioactive and stable cesium isotope concentrations in all compartments of the ecosystem have not been reached yet. However, in some compartments the correlation is already strong. An increase of radiocesium concentrations in young foliage in 2016, compared to 2015, and an increase in 2015-2016 of the 137 Cs/ 133 Cs concentration ratio in the biomass compartments with strong correlations indicate an increase in root uptake of radiocesium from the soil profile. Mass balance of the radionuclide inventories, and accounting for radiocesium fluxes in litterfall, throughfall and stemflow, enabled a rough estimate of the annual radiocesium root uptake flux as 2 ± 1% of the total inventory in the ecosystem

Radioactive ion beam facilities in Europe

International Nuclear Information System (INIS)

Blumenfeld, Y.

2008-01-01

The past two decades have seen extraordinarily rapid development of radioactive beam physics throughout the world and in particular in Europe. The important scientific advances have stemmed from a large number of facilities. Previously existing stable beam machines have been adapted to produce rare isotope beams and dedicated facilities have come on-line. This talk gives an overview of the present European installations highlighting their complementary nature. The European roadmap calls for the construction of two next generation facilities: FAIR making use of projectile fragmentation and EURISOL based on the ISOL technique. The future FAIR facility will be described and the path towards EURISOL presented in the light of the construction of 'intermediate' generation facilities SPIRAL2, HIE ISOLDE and SPES and results from the ongoing EURISOL Design Study.

Radioactive Materials in Medical Institutions as a Potential Threat

International Nuclear Information System (INIS)

Radalj, Z.

2007-01-01

In numerous health institutions ionizing sources are used in everyday practice. Most of these sources are Roentgen machines and accelerators which produce radiation only when in use. However, there are many institutions, e.g., Nuclear medicine units, where radioactive materials are used for diagnostic and therapeutic purposes. This institutions store a significant amount of radioactive materials in form of open and closed sources of radiation. Overall activity of open radiation sources can reach over a few hundred GBq. Open sources of radiation are usually so called short-living isotopes. Since they are used on daily basis, a need for a continuous supply of the radioactive materials exists (on weekly basis). Transportation phase is probably the most sensitive phase because of possible accidents or sabotage. Radiological terrorism is a new term. Legislation in the area of radiological safety is considered complete and well defined, and based on the present regulatory mechanism, work safety with radiation sources is considered relatively high. However, from time to time smaller accidents do happen due to mishandling, loose of material (possible stealing), etc. Lately, the safety issue of ionizing sources is becoming more important. In this matter we can expect activities in two directions, one which is going towards stealing and 'smuggling' of radioactive materials, and the other which would work or provoke accidents at the location where the radiation sources are.(author)

Sulfur Isotope Exchange between S-35 Labeled Inorganic Sulfur-Compounds in Anoxic Marine-Sediments

DEFF Research Database (Denmark)

FOSSING, H.; THODEANDERSEN, S.; JØRGENSEN, BB

1992-01-01

of isotope exchange, specific radioactivities of the reduced sulfur pools were poorly defined and could not be used to calculate their rates of formation. Such isotope exchange reactions between the reduced inorganic sulfur compounds will affect the stable isotope distribution and are expected to decrease...

Production, administration and disposal of cyclotron produced shortlived radioactive gases for positron emission tomography studies at the Austin Repatriation Medical Centre, Melbourne

Energy Technology Data Exchange (ETDEWEB)

Egan, G.F.; O`Keefe, G. [Austin Hospital, Heidelberg, VIC (Australia); Tochon-Danguy, H.J.; Midgley, S.; Phana, K.S.; Sachinidis, J.; Chan, J.G. [Melbourne Univ., Parkville, VIC (Australia). School of Physics

1995-01-01

Positron Emission Tomography (PET) Centre is operational at the Austin Repatriation Medical Centre, Melbourne. The major equipment consists of a 10 MeV cyclotron and a whole body PET scanner. Radioactive gases produced and used directly in clinical studies include [{sup 15}O]O{sub 2}, [{sup 15}O]CO, and [{sup 15}O]CO{sub 2}, whilst [{sup 11}C]CO{sub 2} is also produced for use in radiochemistry syntheses. Radioactivity delivery rates of 3.7, 3.3, and 1.6 GBq/min to the scanner suite have been achieved for [{sup 15}O]O{sub 2}, [{sup 15}O]CO{sub 2}, and [{sup 15}O]CO respectively, and batch productions of 36.3 GBq of [{sup 11}C]CO{sub 2} have been produced. The production. patient administration and disposal of the short-lived radioactive gases has been achieved in compliance with radiation protection principles. Radioactive gas doses of 1.7 GBq are administered to patients with less than 0.02 MBq/m{sup 3} leakage into the scanner suite. Less than 13 MBq of [ {sup 15}O]-labelled gases are released into the environment per patient study at a concentration of 0.018 MBq/m{sup 3}. Annually less than 2 GBq is expected to be released into the environment. The centre design and first four months` experience of radioactive gas production, administration and disposal is presented. 5 refs., 4 tab., 1 fig.

A Time-Measurement System Based on Isotopic Ratios

International Nuclear Information System (INIS)

Vo, Duc T.; Karpius, P.J.; MacArthur, D.W.; Thron, J.L.

2007-01-01

A time-measurement system can be built based on the ratio of gamma-ray peak intensities from two radioactive isotopes. The ideal system would use a parent isotope with a short half-life decaying to a long half-life daughter. The activities of the parent-daughter isotopes would be measured using a gamma-ray detector system. The time can then be determined from the ratio of the activities. The best-known candidate for such a system is the 241 Pu- 241 Am parent-daughter pair. However, this 241 Pu- 241 Am system would require a high-purity germanium detector system and sophisticated software to separate and distinguish between the many gamma-ray peaks produced by the decays of the two isotopes. An alternate system would use two different isotopes, again one with a short half-life and one with a half-life that is long relative to the other. The pair of isotopes 210 Pb and 241 Am (with half-lives of 22 and 432 years, respectively) appears suitable for such a system. This time-measurement system operates by measuring the change in the ratio of the 47-keV peak of 210 Pb to the 60-keV peak of 241 Am. For the system to work reasonably well, the resolution of the detector would need to be such that the two gamma-ray peaks are well separated so that their peak areas can be accurately determined using a simple region-of-interest (ROI) method. A variety of detectors were tested to find a suitable system for this application. The results of these tests are presented here.

Isotopic separation

International Nuclear Information System (INIS)

Chen, C.L.

1982-01-01

A method is described for separating isotopes in which photo-excitation of selected isotope species is used together with the reaction of the excited species with postive ions of predetermined ionization energy, other excited species, or free electrons to produce ions or ion fragments of the selected species. Ions and electrons are produced by an electrical discharge, and separation is achieved through radial ambipolar diffusion, electrostatic techniques, or magnetohydrodynamic methods

The management of radioactive wastes produced by medical institutions in Japan

International Nuclear Information System (INIS)

Kikuchi, Akira

1981-01-01

The use of radiopharmaceuticals is faced with rather dark prospects. The reason is that the management of radioactive wastes does not work smoothly. In the present management system for low level radioactive wastes in Japan, the Japan Radioisotope Association (JRIA) plays the part of collecting them and the Japan Atomic Energy Research Institute (JAERI) plays that of treating them. The volume of radioactive wastes collected, however, is far greater than that treated. Correspondingly, JRIA has to store the excessive radioactive wastes. The construction of a new treatment facility is urgently needed and the search for a building lot goes on. All those concerned, the users and suppliers of radiopharmaceuticals, and so on, should be aware of the situation and cooperate to resolve the various problems concerning the management of radioactive wastes generated by themselves. (author)

The role of chemistry in the history of radioactivity (1897-1939)

International Nuclear Information System (INIS)

Adloff, J.P.

1997-01-01

Chemical research on radioactivity started in 1898. That year, Pierre and Marie Curie discovered in pitchblende polonium and radium. Rutherford and Soddy showed that radioactivity is an atomic phenomenon accompanied by transmutation of elements and established the basic laws of radioactive changes. The existence of isotopes was postulated after the discovery of many radioactive substances. Major discoveries in nuclear science, i.e. the atomic nucleus, the neutron and artificial radioactivity, were made with radiation sources elaborated bu chemists. Finally, in 1939, radiochemists on the search for transuranium elements, discovered nuclear fission. (authors)

Substantiation of the permissible radioactive contamination of working clothes

International Nuclear Information System (INIS)

Shcherbakov, V.L.; Korostin, A.S.

1977-01-01

A permissible level of working clothes contamination was determined on the base of the main migration routes of radioactive contaminants: permeation directly through the clothes into subclothes space on skin surface, emission into the air with amount of contaminants subsequently got by the organism of a working person through inhalation as well as transfer in the process of contacting of contaminated working clothes and surfaces of premises equipment, working person hands with amount of contaminants posteriorly got by the organism by alimentary or inhalation ways. Using the experimental and literature data available the permissible levels of working clothes contamination for the mentioned migration routes of radioactive materials have been calculated. According to the data obtained the permissible levels of working clothes contamination must not exceed 4 alpha-part/(cm 2 xmin) for contamination with high-tonic isotopes, 20 alpha-part./(cm 2 xmin) with other alpha-detine isotopes, 1000 beta-part./(cm 2 xmin) with beta-active ones. The permissible level of contamination of additional materials of the individual protection in the case of their contamination with high-tonic alpha-actine isotopes must not exceed 50 alpha-part./(cm 2 xmin), 200 alpha-part./(cm 2 xmin) for contamination th other alpha-active isotopes and 400 beta-part./(cm 2 xmin) with beta-active isotopes

On line isotopic separator test benches at GANIL

International Nuclear Information System (INIS)

Anne, R.; Bru, B.; Joubert, A.; Leroy, R.; Obert, J.; Putaux, J.C.; Liang, C.F.; Paris, P.; Orr, N.; Steckmeyer, J.C.

1993-01-01

A first version of isotopic separator on line test bench has been built in order to test the feasibility of the production of radioactive species from 96 MeV/u of 20 Ne impinging a thick target of MgO. This test bench was equipped with a very compact ECR ion source (Nanogan) entirely made from permanent magnets and operating at 10 Ghz. 18 Ne 2,4+ ; 19N e 1,2,3,4+ and 23,24 Ne 1+ has been produced and ionized. A new more performing separator (SIRa) allowing the use of different types of ion sources will be completed by the end of 1993. (author) 4 refs., 4 figs., 1 tab

Long lived isotopes in the Chernobyl radioactive cloud at Cracow

International Nuclear Information System (INIS)

Mietelski, J.W.; Broda, R.; Sieniawski, J.

1988-01-01

The analysis of the residual gamma radioactivity in the air filters exposed during the passage of the Chernobyl radioactive cloud over Cracow area gave data on variation in time of the relative contribution of long lived radioisotopes. Conclusions on transport properties of some elements are deduced from the obtained results. 10 refs., 5 figs. (author)

Isotopic characterization as a screening tool in authentication of organic produce commercially available in western North America.

Science.gov (United States)

Verenitch, Sergei; Mazumder, Asit

2015-01-01

The use of nitrogen stable isotopes to discriminate between conventionally and organically grown crops has been further developed in this study. Soil and irrigation water from different regions, as well as nitrogen fertilizers used, have been examined in detail to determine their effects on nitrogen isotope composition of spinach, lettuce, broccoli and tomatoes. Over 1000 samples of various types of organically and conventionally grown produce of known origin, along with the samples of nitrogen fertilizers used for their growth, have been analysed in order to assemble the datasets of crop/fertilizer correlations. The results demonstrate that the developed approach can be used as a valuable component in the verification of agricultural practices for more than 25 different types of commercially grown green produce, either organic or conventional. Over a period of two years, various organic and non-organic greens, from different stores in Seattle (WA, USA) and Victoria (BC, Canada), were collected and analysed using this methodology with the objective of determining any pattern of misrepresentation.

Project requirements for reconstruction of the RA reactor ventilation system, Task 2.8. Measurement of radioactive iodine and other isotopes contents in the gas system of the RA reactor, Annex of the task

International Nuclear Information System (INIS)

Vujisic, Lj. et al

1981-01-01

This report is a supplement to the task 2.8. When planning and constructing the ventilation system, it was found that it is necessary to perform additional experiments during RA reactor operation at 2 MW power level for a longer period. In addition to the helium system, the potential source of radioactive pollutants is the space below the upper water shielding of the reactor. All the experimental and fuel channels are ending in this space. During repair and fuel exchange radioactivity can be released in this space. For that reason this space is important when planing and designing the filtration system for incidental conditions or planned dehermetisation of the reactor. The third point where radioactive isotope identification was done, was the entrance into the chimney during steady state operation and planned dehermetisation of the reactor. The following samples were measured: gas system during reactor operation at 2 MW power; entrance into the chimney during last 48 hours of reactor operation at 2 MW power; sample on the platform under the upper water shield with the opened fuel channel after the reactor shutdown; and simultaneously with the latter, measurement at the entrance to the chimney. This annex contains the list of identified radioactive isotopes, volatile and gaseous as well as concentration of volatile 131 I on the adsorbents [sr

Selected research works published in international journals on Vietnam environmental radioactivity

International Nuclear Information System (INIS)

2012-01-01

The environmental radioactivity is object of many studies of the Vietnam Atomic Energy Institute (VINATOM). The VINATOM for long time has carried out monitoring of environmental radioactivity and application of isotopes in investigation of natural resources for socio-economic development in Vietnam. A lot of results of the studies in monitoring and application of radiation and isotopes have been presented at conferences. Some excellent research works have been published in prestigious international journals and selected to republish in this collection. The publication is expected to be as reference material for researchers, postgraduates in the field of environment protection. (NHA)

Penning-trap mass measurements of exotic rubidium and gold isotopes for a mean-field study of pairing and quadrupole correlations

CERN Document Server

Manea, Vladimir

2015-09-14

The most complex nuclei are situated between the magic and the mid-shell ones, in regions known for sudden changes of the trends of nuclear observables. These are the so-called shape-transition regions, where the nuclear paradigm changes from the vibrational liquid drop to the static rotor. With few exceptions, nuclei in these regions are radioactive, with half-lives dropping into the millisecond range. Complementing the information obtained from the low-lying excitation spectrum, nuclear binding energies and mean-square charge radii are among the observables most sensitive to these changes of nuclear structure. In the present work, a study of the shape- transition phenomenon is performed by measurements of radioactive nuclides produced by the ISOLDE facility at CERN. The masses of the neutron-rich rubidium isotopes $^{98-100}$Rb and of the neutron-deficient gold isotopes $^{180, 185, 188, 190, 191}$Au are determined using the Penning-trap mass spectrometer ISOLTRAP. The mass of $^{100}$Rb is determined for t...

Regulation of naturally occurring and accelerator-produced radioactive materials: an update

International Nuclear Information System (INIS)

Bolling, L.A.; Lubenau, J.O.; Nussbaumer, D.A.

1984-10-01

In 1977, NRC published a report (NUREG-0301) of a task force review of the need for, and feasibility of, the Federal government regulating naturally occurring and accelerator-produced radioactive materials (NARM). Since that time, the Federal regulatory role has not significantly changed but State calls for increased Federal involvment have continued. In 1983, a National Governors' Association report on the NRC Agreement State program recommended amendment of the Atomic Energy Act to authorize NRC regulation of these materials. Based on that recommendation, and with the cooperation of the Conference of Radiation Control Program Directors, Inc., NRC staff undertook a review of the current status of use and regulation of NARM. This report contains the results of that review. 10 references

Concentration of caesium isotopes in foodstuffs in Poland

International Nuclear Information System (INIS)

Grabowski, D.; Rubel, B.; Muszynski, W.; Kurowski, W.; Swietochowska, J.; Smagala, G.

2000-01-01

One of the sources of the radioactive doses obtained by people resulting from the radiological contamination of the environment, is the transfer of radionuclides to the organism via ingestion. Radioactive isotopes in foodstuffs appear as a result of nuclear activities on the globe, mainly because of nuclear explosion and, recently, after the Chernobyl accident. Since the early sixties the network of Service for Measurement of Radioactive Contamination in Poland systematically controlled all kinds of important food products. Radiochemical methods and gamma spectrometry has been used to determination the activity of radioactive isotopes. This contribution reports of the determination of 134 Cs and 137 Cs concentration in milk, meat, vegetables, fruits, cereals and 'forest products' during period 1985-1999. In 1985 the average 137 Cs level was below 1 Bq/kg (except forest products). Moreover, no regional differences were observed the whole territory of Poland. After the Chernobyl accident situation changed completely. Average activity of 137 Cs in milk was 25 Bq/l in May 1986, 20-25 Bq/kg in beef and 10-15 Bq/kg in pork (summer months). Also fruit picked up in June and July was contaminated, mainly currents. The contamination of vegetables was less important. The activity of cesium isotopes in forest mushrooms and wild game were much higher than in other tested foodstuffs. From the 1987 level of radioactive contamination was decreasing gradually. In 1999 the activity of 137 Cs of vegetables, cereals, fruit was on level as it has been in 1985 as for meat and milk it is higher. Level of radiocesium in 'forest products' is still high. The average annual effective dose from ingestion of radiocesium was on level 0.088 mSv in 1986 and 0.006 mSv in 1999. (author)

Health risk assessment for radium discharged in produced waters

International Nuclear Information System (INIS)

Hamilton, L.D.; Meinhold, A.F.; Nagy, J.

1991-01-01

Produced water generated during the production of oil and gas can contain enhanced levels of radium. This naturally occurring radioactive material (NORM) is discharged into freshwater streams, estuarine, coastal and outer continental shelf waters. Large volumes of produced waters are discharged to coastal waters along the Gulf Coast of Louisiana. The Gulf of Mexico is an important producer of fish and shellfish, and there is concern that radium discharged to coastal Louisiana could contaminate fish and shellfish used by people for food, and present a significant increase in cancer risk. This paper describes a screening-level assessment of the potential cancer risks posed by radium discharged to coastal Louisiana in oil-field produced waters. This screening analysis was performed to determine if a more comprehensive and realistic assessment is necessary, and because of the conservative assumptions embedded in the analysis overestimates the risk associated with the discharge of radium in produced waters. Two isotopes of radium (Ra-226 and Ra-228) are the radionuclides of most concern in produced water in terms of potential human health effects

Possibility of wine dating using the natural Pb-210 radioactive isotope

International Nuclear Information System (INIS)

Hubert, Ph.; Pravikoff, M.S.; Gaye, J.

2015-01-01

To control the authenticity of an old wine without opening the bottle, we developed a few years ago a method based on the measurement of the 137 Cs activity. However, for recent vintages, the 137 Cs activity drops to far too low values (most of the time less than 10 mBq/L for a 10-year-old wine) for this method to perform correctly. In this paper we examine the possibility to date wines using the natural radio-element 210 Pb which has a 22-year period. This new method we propose implies the opening of the bottle and the follow-on destruction of the wine itself, which means that it can only be used for investigating non-expensive bottles or wine lots where there are multiple bottles of the same provenance. Uncertainties on the resulting 210 Pb radioactivity values are large, up to more than 50%, mainly due to local atmospheric variations, which prevents us to carry out precise dating. However it can be used to discriminate between an old wine (pre-1952) and a young wine (past-1990), an information that cannot be obtained with the other techniques based on other isotopes ( 137 Cs, 14 C or tritium). - Highlights: • We correlate the measured 210 Pb activity in wine to the vintage year. • A precise dating with 210 Pb is still difficult. • The method is complementary to the 137 Cs technique we previously developed

Method for the radioactive determination of the foliates

International Nuclear Information System (INIS)

Rosen, H.

1976-01-01

A method is described for the radioactive determination of the foliates, in which a determination is made of the uptake on a protein fraction of the milk taking up the foliates by competition between the foliate(s) to be determined and a folic acid by-product labelled with a radioactive isotope. The characteristics of this method is that it consists in using tyramide of iodinated folic acid 125 [fr

Novel method of producing radioactive iodine

International Nuclear Information System (INIS)

Shikata, E.; Amano, H.

1976-01-01

Radioactive iodine(I-131) is easily obtained by heating, at a temperature ranging from 600 0 C to 650 0 C, a tellurium oxide intermediate which was obtained by heating telluric acid or tellurium trioxide at a temperature from about 400 0 C to 560 0 C and was irradited with a neutron flux. Thus, pure I-131 is obtained without the complicated operations required in a conventional process for separation and/or purification of the product. 4 claims

Isotope production

Energy Technology Data Exchange (ETDEWEB)

Lewis, Dewi M.

1995-07-15

Some 2 0% of patients using radiopharmaceuticals receive injections of materials produced by cyclotrons. There are over 200 cyclotrons worldwide; around 35 are operated by commercial companies solely for the production of radio-pharmaceuticals with another 25 accelerators producing medically useful isotopes. These neutron-deficient isotopes are usually produced by proton bombardment. All commonly used medical isotopes can be generated by 'compact' cyclotrons with energies up to 40 MeV and beam intensities in the range 50 to 400 microamps. Specially designed target systems contain gram-quantities of highly enriched stable isotopes as starting materials. The targets can accommodate the high power densities of the proton beams and are designed for automated remote handling. The complete manufacturing cycle includes large-scale target production, isotope generation by cyclotron beam bombardment, radio-chemical extraction, pharmaceutical dispensing, raw material recovery, and labelling/packaging prior to the rapid delivery of these short-lived products. All these manufacturing steps adhere to the pharmaceutical industry standards of Good Manufacturing Practice (GMP). Unlike research accelerators, commercial cyclotrons are customized 'compact' machines usually supplied by specialist companies such as IBA (Belgium), EBCO (Canada) or Scanditronix (Sweden). The design criteria for these commercial cyclotrons are - small magnet dimensions, power-efficient operation of magnet and radiofrequency systems, high intensity extracted proton beams, well defined beam size and automated computer control. Performance requirements include rapid startup and shutdown, high reliability to support the daily production of short-lived isotopes and low maintenance to minimize the radiation dose to personnel. In 1987 a major step forward in meeting these exacting industrial requirements came when IBA, together with the University of Louvain-La-Neuve in Belgium, developed the Cyclone-30

Radioactivity in man

International Nuclear Information System (INIS)

Syed, I.B.

1979-01-01

An account of the various radioisotopes present in the human body, such as the naturally occurring isotopes 40 K, 14 C etc. is given. Other harmful isotopes such as radiophosphorus 32 P, 90 Sr, 87 Rb, 45 Ca, 137 Ce, 131 I and tritium which find their way into the human system either by accidental ingestion or from fallout or during radiodiao.nosis or therapy are also discussed. 90 Sr which has a half-life of 28 years and can enter the human body through milk and other animal foods, is dealt with in detail, because of its being a pure beta emitter. Other general radioactive hazards to the human population in the world are also touched upon. (K.B.)

Lead isotope in mineral exploration

International Nuclear Information System (INIS)

Gulson, B.L.

1986-01-01

This book provides an up-to-date state-of-the-art review of lead isotopes in mineral exploration. Beginning with an historical review on suggested uses of lead isotopes in mineral exploration, the author then outlines the theoretical aspects of lead isotopes and illustrates that the method is based on well-known principles of radioactive decay, from which isotopic signatures for different styles of mineralization are derived. The varying isotopic signatures are then introduced. The major part of the book details over 40 case histories for base and precious metals, uranium and tin using sampling media such as sulfides, gossans, soils, weathered bedrock, vegetation and groundwaters. Advantages and disadvantages of each are discussed. Examples are given of the use of lead isotopes in testing conceptual models for exploration. The success rate and cost-effectiveness of the method are illustrated by actual exploration examples. Analytical advances which should lower the cost of the method and future uses are outlined. Many of the case histories use recently published or unpublished data, 27 tables of which are given in an appendix. Details of sampling, the methods for obtaining the isotope ratios, and a commercially-available integrated lead isotope service are also provided. (Auth.)

Isotopic techniques in radioactive waste disposal site evaluation: a method for reducing uncertainties I. T, T/3He, 4He, 14C, 36Cl

International Nuclear Information System (INIS)

Muller, A.B.

1981-01-01

This paper introduces five of the isotopic techniques which can help reduce uncertainties associated with the assessment of radioactive waste disposal sites. The basic principles and practical considerations of these best known techniques have been presented, showing how much additional site specific information can be acquired at little cost or consequence to containment efficiency. These methods, and the more experimental methods appearing in the figure but not discussed here, should be considered in any detailed site characterization, data collection and analysis

Study of the radioactivity of the lower Danube during the period 1970-1974

International Nuclear Information System (INIS)

Iorgulescu, A.; Iorgulescu, St.; Rogalski, I.

1975-01-01

The control of radioactive pollution of the inferior course of Danubian river is perform in this paper. The results achieved by spectroscopic analyse of the samples of water, sediment and vegetation has indicated that; gamma radioactivity, beta radioactivity and isotopic concentration in tritium U-238, Th-232, Pb-212, Ra-226, potassium-40 is below superior limit admitted

Storage of radioactive waste

International Nuclear Information System (INIS)

Pittman, F.K.

1974-01-01

Four methods for managing radioactive waste in order to protect man from its potential hazards include: transmutation to convert radioisotopes in waste to stable isotopes; disposal in space; geological disposal; and surface storage in shielded, cooled, and monitored containers. A comparison of these methods shows geologic disposal in stable formations beneath landmasses appears to be the most feasible with today's technology. (U.S.)

Reconstruction of the isotope activity content of heterogeneous nuclear waste drums.

Science.gov (United States)

Krings, Thomas; Mauerhofer, Eric

2012-07-01

Radioactive waste must be characterized in order to verify its conformance with national regulations for intermediate storage or its disposal. Segmented gamma scanning (SGS) is a most widely applied non-destructive analytical technique for the characterization of radioactive waste drums. The isotope specific activity content is generally calculated assuming a homogeneous matrix and activity distribution for each measured drum segment. However, real radioactive waste drums exhibit non-uniform isotope and density distributions most affecting the reliability and accuracy of activities reconstruction in SGS. The presence of internal shielding structures in the waste drum contributes generally to a strong underestimation of the activity and this in particular for radioactive sources emitting low energy gamma-rays independently of their spatial distribution. In this work we present an improved method to quantify the activity of spatially concentrated gamma-emitting isotopes (point sources or hot spots) in heterogeneous waste drums with internal shielding structures. The isotope activity is reconstructed by numerical simulations and fits of the angular dependent count rate distribution recorded during the drum rotation in SGS using an analytical expression derived from a geometric model. First results of the improved method and enhancements of this method are shown and are compared to each other as well as to the conventional method which assumes a homogeneous matrix and activity distribution. It is shown that the new model improves the accuracy and the reliability of the activity reconstruction in SGS and that the presented algorithm is suitable with respect to the framework requirement of industrial application. Copyright © 2011 Elsevier Ltd. All rights reserved.