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Sample records for quasielastic neutron scattering

  1. Quasielastic neutron scattering facility at Dhruva reactor

    International Nuclear Information System (INIS)

    Mukhopadhyay, R.; Mitra, S.; Paranjpe, S.K.; Dasannacharya, B.A.

    2001-01-01

    Quasi-elastic neutron scattering is a powerful experimental tool for studying the various dynamical motions in solids and liquids. In this paper, we have described the salient features of the quasi-elastic neutron spectrometer in operation at Dhruva reactor at Trombay, India. The design criteria have been such as to maximise the throughput by various means like closer approach to the source, focusing a larger beam on to a sample, and Multi-Angle Reflecting X-tal mode of energy analysis. Some results of molecular motions from recently studied systems using this spectrometer are also reported

  2. Molecular dynamics using quasielastic neutron scattering

    CERN Document Server

    Mitra, S

    2003-01-01

    Quasielastic neutron scattering (QENS) technique is well suited to study the molecular motions (rotations and translations) in solids or liquids. It offers a unique possibility of analysing spatial dimensions of atomic or molecular processes in their development over time. We describe here some of the systems studied using the QENS spectrometer, designed, developed and commissioned at Dhruva reactor in Trombay. We have studied a variety of systems to investigate the molecular motion, for example, simple molecular solids, molecules adsorbed in confined medium like porous systems or zeolites, monolayer-protected nano-sized metal clusters, water in Portland cement as it cures with time, etc. (author)

  3. Incoherent quasielastic neutron scattering from plastic crystals

    International Nuclear Information System (INIS)

    Bee, M.; Amoureux, J.P.

    1980-01-01

    The aim of this paper is to present some applications of a method indicated by Sears in order to correct for multiple scattering. The calculations were performed in the particular case of slow neutron incoherent quasielastic scattering from organic plastic crystals. First, an exact calculation (up to second scattering) is compared with the results of a Monte Carlo simulation technique. Then, an approximation is developed on the basis of a rotational jump model which allows a further analytical treatment. The multiple scattering is expressed in terms of generalized structure factors (which can be regarded as self convolutions of first order structure factors taking into account the instrumental geometry) and lorentzian functions the widths of which are linear combinations of the jump rates. Three examples are given. Two of them correspond to powder samples while in the third we are concerned with the case of a single crystalline slab. In every case, this approximation is shown to be a good approach to the multiple scattering evaluation, its main advantage being the possibility of applying it without any preliminary knowledge of the correlation times for rotational jumps. (author)

  4. Quasielastic neutron scattering in biology: Theory and applications.

    Science.gov (United States)

    Vural, Derya; Hu, Xiaohu; Lindner, Benjamin; Jain, Nitin; Miao, Yinglong; Cheng, Xiaolin; Liu, Zhuo; Hong, Liang; Smith, Jeremy C

    2017-01-01

    Neutrons scatter quasielastically from stochastic, diffusive processes, such as overdamped vibrations, localized diffusion and transitions between energy minima. In biological systems, such as proteins and membranes, these relaxation processes are of considerable physical interest. We review here recent methodological advances and applications of quasielastic neutron scattering (QENS) in biology, concentrating on the role of molecular dynamics simulation in generating data with which neutron profiles can be unambiguously interpreted. We examine the use of massively-parallel computers in calculating scattering functions, and the application of Markov state modeling. The decomposition of MD-derived neutron dynamic susceptibilities is described, and the use of this in combination with NMR spectroscopy. We discuss dynamics at very long times, including approximations to the infinite time mean-square displacement and nonequilibrium aspects of single-protein dynamics. Finally, we examine how neutron scattering and MD can be combined to provide information on lipid nanodomains. This article is part of a Special Issue entitled "Science for Life" Guest Editor: Dr. Austen Angell, Dr. Salvatore Magazù and Dr. Federica Migliardo. Copyright © 2016 Elsevier B.V. All rights reserved.

  5. Quasielastic Neutron Scattering by Superionic Strontium Chloride

    DEFF Research Database (Denmark)

    Dickens, M. H.; Hutchings, M. T.; Kjems, Jørgen

    1978-01-01

    The scattering, from powder and single crystal samples, appears only above the superionic transition temperature, 1000K. The integrated intensity is found to be strongly dependent on the direction and magnitude of the scattering vector, Q, (which suggests the scattering is coherent) but does not ...

  6. Quasielastic neutron scattering and microscopic dynamics of liquid ethylene glycol

    Energy Technology Data Exchange (ETDEWEB)

    Sobolev, O. [Laboratoire de Geophysique Interne et Tectonophysique, BP 53, Maison des Geosciences - Domaine Universitaire, 38041 Grenoble, Cedex 9 (France)], E-mail: Oleg.Sobolev@ujf-grenoble.fr; Novikov, A. [Institute for Physics and Power Engineering, Bondarenko Sq. 1, Obninsk, Kaluga Reg. 249033 (Russian Federation); Pieper, J. [Technische Universitaet Berlin, Strasse des 17, Juni 135, D-10623 Berlin (Germany)

    2007-04-20

    Quasielastic neutron scattering (QENS) by liquid ethylene glycol was analyzed using different model approaches. It was found that approximation of the QENS spectra by a set of Lorentzian functions corresponding to the translational and rotational motions produce physically unrealistic results. At the same time, the Fourier transform of the stretched-exponential function exp(-(t/{tau}){sup {beta}}) fits the experimental data well, and results of the fit are in good agreement with those obtained earlier for other systems. The stretching parameter {beta} was found Q independent and shows weak temperature dependence. The mean relaxation time as a function of Q departs strongly from the simple diffusion low and can be approximated by a power law <{tau}{sub w}> = {tau}{sub 0}Q{sup -{gamma}} with the exponent parameter {gamma} = 2.4.

  7. A quasi-elastic neutron scattering and neutron spin-echo study of hydrogen bonded system

    Energy Technology Data Exchange (ETDEWEB)

    Branca, C.; Faraone, A.; Magazu, S.; Maisano, G.; Mangione, A

    2004-07-15

    This work reports neutron spin echo results on aqueous solutions of trehalose, a naturally occurring disaccharide of glucose, showing an extraordinary bioprotective effectiveness against dehydration and freezing. We collected data using the SPAN spectrometer (BENSC, Berlin) on trehalose aqueous solutions at different temperature values. The obtained findings are compared with quasi-elastic neutron scattering results in order to furnish new results on the dynamics of the trehalose/water system on the nano and picoseconds scale.

  8. Note on some quasielastic neutron scattering analysis programs on the Rutherford Laboratory IBM 360/195

    International Nuclear Information System (INIS)

    Richardson, R.M.

    1979-12-01

    A suite of programs for analysing neutron scattering data from time-of-flight spectrometers has been implemented on the Rutherford Laboratory IBM 360/195 computer system. The programs are intended for near inelastic and quasielastic data and operate by convoluting the measured instrumental resolution function with a model scattering function before fitting to the measured sample scattering law. (author)

  9. Proton dynamics in oxides: insight into the mechanics of proton conduction from quasielastic neutron scattering.

    Science.gov (United States)

    Karlsson, Maths

    2015-01-07

    This article is concerned with the use of quasielastic neutron scattering as a technique for investigation of the dynamical properties of proton conducting oxides. Currently, the main interest in these materials comes from their promise as electrolytes in future electrochemical devices and particularly through their use as electrolytes in next-generation, intermediate-temperature, fuel cells. However, the realization of such devices depends critically on the development of new, more highly proton conducting oxides. Such a development depends on increasing the current understanding of proton conduction in oxides and for this purpose quasielastic neutron scattering is an important mean. The aim of this article is to introduce the non-specialist reader to the basic principles of quasielastic neutron scattering, its advantages and disadvantages, to summarize the work that has been done on proton conducting oxides using this technique, as well as to discuss future opportunities within this field of research.

  10. Interpretation of the quasi-elastic neutron scattering on PAA by rotational diffusion models

    International Nuclear Information System (INIS)

    Bata, L.; Vizi, J.; Kugler, S.

    1974-10-01

    First the most important data determined by other methods for para azoxy anisolon (PAA) are collected. This molecule makes a rotational oscillational motion around the mean molecular direction. The details of this motion can be determined by inelastic neutron scattering. Quasielastic neutron scattering measurements were carried out without orienting magnetic field on a time-of-flight facility with neutron beam of 4.26 meV. For the interpretation of the results two models, the spherical rotation diffusion model and the circular random walk model are investigated. The comparison shows that the circular random walk model (with N=8 sites, d=4A diameter and K=10 10 s -1 rate constant) fits very well with the quasi-elastic neutron scattering, while the spherical rotational diffusion model seems to be incorrect. (Sz.N.Z.)

  11. Incoherent quasielastic neutron scattering from water in supercooled regime

    International Nuclear Information System (INIS)

    Chen, S.; Teixeira, J.; Nicklow, R.

    1982-01-01

    Measurements of the quasielastic spectra have been made with a three-axis neutron spectrometer at constant-Q mode in a temperature range from 38 0 C down to -20 0 C. Two energy resolutions both high (δE = 100 μ eV) and low (δE = 800 μ eV) were used to identify and separate a sharp component from a broad one. As temperature is decreased below zero the spectrum shows an increasing sharp component standing out on top of the broad one. The broad component is attributed to rotational motions of water molecules. A preliminary analysis of the linewidths gives a Q-independent relaxation time which has the same magnitude as the rotational relaxation time measured by nuclear magnetic resonance. The Q dependence of the sharp line is analyzed by a Q-dependent diffusion coefficient. A temperature-independent characteristic length l 0 = 0.5 A is obtained. We then attempt to relate this length to local geometry of protons associated with hydrogen bonding

  12. Inelastic and quasielastic neutron scattering studies on soft matter and biomolecules

    International Nuclear Information System (INIS)

    Kanaya, Toshiji

    2015-01-01

    Some characteristic features of soft matter and biomolecules in the inelastic and quasielastic neutron scattering (INS and QENS) studies are described. In order to clarify the current situation of the studies the research history on soft matter and biomolecules by INS and QENS are described. As examples of the studies of slow dynamics of soft matter, neutron spin echo studies on breathing mode of polymer micelle and static and dynamics fluctuations in polymer gels. (author)

  13. Ion conducting behavior in secondary battery materials detected by quasi-elastic neutron scattering measurements

    International Nuclear Information System (INIS)

    Nozaki, Hiroshi

    2014-01-01

    Ionic conducting behaviors in secondary battery materials, i.e. cathode and solid electrolyte, were studied with quasi-elastic neutron scattering (QENS) measurements. Although the incoherent scattering length for Li and Na is lower by two orders of magnitude than that for H, the QENS spectra were clearly detected using the combination of an intense neutron source and a low background spectrometer. The fundamental parameters, such as, the activation energy, the jump distance, and the diffusion coefficient were obtained by analyzing QENS spectra. These parameters are consistent with the previous results estimated by muon-spin relaxation (μSR) measurements and first principles calculations. (author)

  14. Study of the diffusion movements of water by quasi-elastic scattering of slow neutrons

    International Nuclear Information System (INIS)

    Yamazaki, Ione Makiko

    1980-01-01

    The diffusion movements of water at three different temperatures in the liquid state have been studied by slow neutron quasi-elastic scattering. The measurements have been performed using the IPEN Triple Axis Spectrometer. Broadening and integrated intensity of the quasi-elastic line have been determined for several momentum transfer (K) in the range 0,7627 ≤ K ≤ 2,993 A -1 . The broadening of the quasi-elastic peaks as function of momentum transfer (K) observed at various temperatures has been interpreted in terms of globular diffusion models. The results obtained at 30 deg C have been explained in a consistent way considering the translational and rotational globular diffusion movements. To describe the results obtained at 55 deg and 70 deg C only the translational globular diffusion model was sufficient. This analysis indicates the existence in water of globules with distance of the farest proton position to the center of gravity of the globule 4,5 A, corroborating the idea of quasi-crystalline structure for water. The Debye-Waller factor has been obtained through the analysis of the integrated intensity of quasi-elastic scattering peaks over the K 2 measured range. From this analysis an estimative of the mean square displacement was obtained. (author)

  15. Analysis of the Quasi-Elastic Scattering of Neutrons in Hydrogenous Liquids

    International Nuclear Information System (INIS)

    Porohit, S.N.

    1966-11-01

    A critical discussion of the quasi-elastic scattering of neutrons by incoherent (hydrogenous) liquids is presented. Using the line shape expression a comparative discussion of several phenomenological models has been carried out. Extension of the Singwi-Sjoelander zero phonon expression, for the jump-diffusion model, so as to include the one phonon expression has also been given. For a delayed diffusion model a complete treatment of S(K, ω) is presented. Along the lines of the macroscopic diffusion cooling, a microscopic diffusion cooling effect in fluids is speculated

  16. Analysis of the Quasi-Elastic Scattering of Neutrons in Hydrogenous Liquids

    Energy Technology Data Exchange (ETDEWEB)

    Porohit, S N [Nuclear Science and Engineering Dept., Rensselaer Polytechnique Inst., Troy, NY (United States)

    1966-11-15

    A critical discussion of the quasi-elastic scattering of neutrons by incoherent (hydrogenous) liquids is presented. Using the line shape expression a comparative discussion of several phenomenological models has been carried out. Extension of the Singwi-Sjoelander zero phonon expression, for the jump-diffusion model, so as to include the one phonon expression has also been given. For a delayed diffusion model a complete treatment of S(K, {omega}) is presented. Along the lines of the macroscopic diffusion cooling, a microscopic diffusion cooling effect in fluids is speculated.

  17. Study of water diffusion on single-supported bilayer lipid membranes by quasielastic neutron scattering

    DEFF Research Database (Denmark)

    Bai, M.; Miskowiec, A.; Hansen, F. Y.

    2012-01-01

    High-energy-resolution quasielastic neutron scattering has been used to elucidate the diffusion of water molecules in proximity to single bilayer lipid membranes supported on a silicon substrate. By varying sample temperature, level of hydration, and deuteration, we identify three different types...... of diffusive water motion: bulk-like, confined, and bound. The motion of bulk-like and confined water molecules is fast compared to those bound to the lipid head groups (7-10 H2O molecules per lipid), which move on the same nanosecond time scale as H atoms within the lipid molecules. Copyright (C) EPLA, 2012...

  18. Quasi-elastic (QENS) and inelastic neutron scattering (INS) on hexamethylbenzene

    Energy Technology Data Exchange (ETDEWEB)

    Krawczyk, J. [H. Niewodniczanski Institute of Nuclear Physics PAN, NZ3, ul. Radzikowskiego 152, 31-342 Cracow (Poland)]. E-mail: jan.krawczyk@ifj.edu.pl; Mayer, J. [H. Niewodniczanski Institute of Nuclear Physics PAN, NZ3, ul. Radzikowskiego 152, 31-342 Cracow (Poland); Natkaniec, I. [H. Niewodniczanski Institute of Nuclear Physics PAN, NZ3, ul. Radzikowskiego 152, 31-342 Cracow (Poland): Frank Laboratory of Neutron Physics, JINR, 141980 Dubna, Russia (Russian Federation); Nowina Konopka, M. [H. Niewodniczanski Institute of Nuclear Physics PAN, NZ3, ul. Radzikowskiego 152, 31-342 Cracow (Poland); Pawlukojc [Frank Laboratory of Neutron Physics, JINR, 141980 Dubna, Russia (RU): Institute of Nuclear Chemistry and Technology, 03-195 Warszawa (Poland); Steinsvoll, O. [Institute for Energy Technology, 2007 Kjeller (Norway); Janik, J.A. [H. Niewodniczanski Institute of Nuclear Physics PAN, NZ3, ul. Radzikowskiego 152, 31-342 Cracow (Poland)

    2005-05-15

    The Quasi-elastic Neutron scattering (QENS) spectra of polycrystalline hexamethylbenzene (HMB) were measured for temperatures from 10K to room temperature (phase III and phase II) for momentum transfer 1.9A{sup -1}. The Inelastic Neutron scattering (INS) and QENS spectra for momentum transfer 0.5-2.9A{sup -1} were measured at T=20, 100 and 130K for energy transfer up to 200meV. The low-resolution diffraction patterns, used as the phase indicator, were also obtained. In the phase III (below 117K), we see practically no quasi-elastic broadening. In phase II, the broadening changes with the temperature are in good agreement with the Arrhenius law. The estimated activation barrier to reorientation is 6kJ/mol. The fitted mean time between instantaneous 120{sup o} jumps of CH{sub 3} groups changes from 10{sup -11}s at T=130K to 2x10{sup -13}s at room temperature. On the basis of EISF versus momentum transfer dependency it is hardly possible to decide what is the geometry of the reorientation. Both reorientation of the CH{sub 3} groups around the three-fold symmetry axis and reorientation of the whole molecule around the six-fold symmetry axis of the benzene ring could describe our results, the former being more probable. The measured INS spectra are compared with the quantum chemical ab initio calculations performed for an isolated HMB molecule.

  19. Quasi-elastic (QENS) and inelastic neutron scattering (INS) on hexamethylbenzene

    International Nuclear Information System (INIS)

    Krawczyk, J.; Mayer, J.; Natkaniec, I.; Nowina Konopka, M.; Pawlukojc; Steinsvoll, O.; Janik, J.A.

    2005-01-01

    The Quasi-elastic Neutron scattering (QENS) spectra of polycrystalline hexamethylbenzene (HMB) were measured for temperatures from 10K to room temperature (phase III and phase II) for momentum transfer 1.9A -1 . The Inelastic Neutron scattering (INS) and QENS spectra for momentum transfer 0.5-2.9A -1 were measured at T=20, 100 and 130K for energy transfer up to 200meV. The low-resolution diffraction patterns, used as the phase indicator, were also obtained. In the phase III (below 117K), we see practically no quasi-elastic broadening. In phase II, the broadening changes with the temperature are in good agreement with the Arrhenius law. The estimated activation barrier to reorientation is 6kJ/mol. The fitted mean time between instantaneous 120 o jumps of CH 3 groups changes from 10 -11 s at T=130K to 2x10 -13 s at room temperature. On the basis of EISF versus momentum transfer dependency it is hardly possible to decide what is the geometry of the reorientation. Both reorientation of the CH 3 groups around the three-fold symmetry axis and reorientation of the whole molecule around the six-fold symmetry axis of the benzene ring could describe our results, the former being more probable. The measured INS spectra are compared with the quantum chemical ab initio calculations performed for an isolated HMB molecule

  20. Quasielastic neutron scattering and molecular dynamics simulation studies of the melting transition in butane and hexane monolayers adsorbed on graphite

    DEFF Research Database (Denmark)

    Hervig, K.W.; Wu, Z.; Dai, P.

    1997-01-01

    Quasielastic neutron scattering experiments and molecular dynamics (MD) simulations have been used to investigate molecular diffusive motion near the melting transition of monolayers of flexible rod-shaped molecules. The experiments were conducted on butane and hexane monolayers adsorbed...... comparison with experiment, quasielastic spectra calculated from the MD simulations were analyzed using the same models and fitting algorithms as for the neutron spectra. This combination of techniques gives a microscopic picture of the melting process in these two monolayers which is consistent with earlier...... neutron diffraction experiments. Butane melts abruptly to a liquid phase where the molecules in the trans conformation translationally diffuse while rotating about their center of mass. In the case of the hexane monolayer, the MD simulations show that the appearance of quasielastic scattering below T...

  1. Quasi-elastic neutron scattering studies of the diffusion of hydrogen in metals

    Energy Technology Data Exchange (ETDEWEB)

    Ross, D K [Birmingham Univ. (UK). School of Physics and Space Research

    1989-01-01

    Quasi-elastic neutron scattering provides a uniquely detailed way of investigating microscopic models for diffusion in lattice gases. In the present paper we discuss extensions of the original Chudley-Elliott model to cover systems containing high concentrations of interacting particles for both the incoherent and coherent cases. In the former case, the peak width is changed by site blocking and by interactions and its shape is altered by correlation effects between successive jumps. In the coherent case, although interactions introduce different correlation effects, the most important changes are due to the short-range order caused by the interactions. A simple Mean Field theory is described which predicts peak narrowing where the diffuse scattering is at a maximum. Experimental tests of both coherent and incoherent theories are described for the case of {alpha}'NbD{sub x}. (orig.).

  2. Quasi-elastic neutron scattering studies of the diffusion of hydrogen in metals

    International Nuclear Information System (INIS)

    Ross, D.K.

    1989-01-01

    Quasi-elastic neutron scattering provides a uniquely detailed way of investigating microscopic models for diffusion in lattice gases. In the present paper we discuss extensions of the original Chudley-Elliott model to cover systems containing high concentrations of interacting particles for both the incoherent and coherent cases. In the former case, the peak width is changed by site blocking and by interactions and its shape is altered by correlation effects between successive jumps. In the coherent case, although interactions introduce different correlation effects, the most important changes are due to the short-range order caused by the interactions. A simple Mean Field theory is described which predicts peak narrowing where the diffuse scattering is at a maximum. Experimental tests of both coherent and incoherent theories are described for the case of α'NbD x . (orig.)

  3. Dynamics of biopolymers on nanomaterials studied by quasielastic neutron scattering and MD simulations

    Science.gov (United States)

    Dhindsa, Gurpreet K.

    Neutron scattering has been proved to be a powerful tool to study the dynamics of biological systems under various conditions. This thesis intends to utilize neutron scattering techniques, combining with MD simulations, to develop fundamental understanding of several biologically interesting systems. Our systems include a drug delivery system containing Nanodiamonds with nucleic acid (RNA), and two specific model proteins, beta-Casein and Inorganic Pyrophosphatase (IPPase). RNA and nanodiamond (ND) both are suitable for drug-delivery applications in nano-biotechnology. The architecturally flexible RNA with catalytic functionality forms nanocomposites that can treat life-threatening diseases. The non-toxic ND has excellent mechanical and optical properties and functionalizable high surface area, and thus actively considered for biomedical applications. In this thesis, we utilized two tools, quasielastic neutron scattering (QENS) and Molecular Dynamics Simulations to probe the effect of ND on RNA dynamics. Our work provides fundamental understanding of how hydrated RNA motions are affected in the RNA-ND nanocomposites. From the experimental and Molecular Dynamics Simulation (MD), we found that hydrated RNA motion is faster on ND surface than a freestanding one. MD Simulation results showed that the failure of Stokes Einstein relation results the presence of dynamic heterogeneities in the biomacromolecules. Radial pair distribution function from MD Simulation confirmed that the hydrophilic nature of ND attracts more water than RNA results the de-confinement of RNA on ND. Therefore, RNA exhibits faster motion in the presence of ND than freestanding RNA. In the second project, we studied the dynamics of a natively disordered protein beta-Casein which lacks secondary structures. In this study, the temperature and hydration effects on the dynamics of beta-Casein are explored by Quasielastic Neutron Scattering (QENS). We investigated the mean square displacement (MSD) of

  4. Broadband Dielectric Spectroscopy and Quasi-Elastic Neutron Scattering on Single-Ion Polymer Conductors

    Science.gov (United States)

    Soles, Christopher; Peng, Hua-Gen; Page, Kirt; Snyder, Chad; Pandy, Ashoutosh; Jeong, Youmi; Runt, James; NIST Collaboration; Pennsylvania Collaboration

    2011-03-01

    The application of solid polymer electrolytes in rechargeable batteries has not been fully realized after decades of research due to its low conductivity. Dramatic increases of the ion conductivity are needed and this progress requires the understanding of conduction mechanism. We address this topic in two fronts, namely, the effect of plasticizer additives and geometric confinement on the charge transfer mechanism. To this end, we combine broadband dielectric spectroscopy (BDS) to characterize the ion mobility and quasi-elastic neutron scattering (QENS) to quantify segmental motion on a single-ion model polymer electrolyte. Deuterated small molecules were used as plasticizers so that the segmental motion of the polymer electrolyte could be monitored by QENS to understand the mechanism behind the increased conductivity. Anodic aluminum oxide (AAO) membranes with well defined channel sizes are used as the matrix to study the transport of ions solvated in a 1D polymer electrolyte.

  5. Hydrogen rotational and translational diffusion in calcium borohydride from quasielastic neutron scattering and DFT

    DEFF Research Database (Denmark)

    Blanchard, Didier; Riktor, M.D.; Maronsson, Jon Bergmann

    2010-01-01

    Hydrogen dynamics in crystalline calcium borohydride can be initiated by long-range diffusion or localized motion such as rotations, librations, and vibrations. Herein, the rotational and translational diffusion were studied by quasielastic neutron scattering (QENS) by using two instruments...... with different time scales in combination with density functional theory (DFT) calculations. Two thermally activated reorientational motions were observed, around the 2-fold (C2) and 3-fold (C3) axes of the BH4− units, at temperature from 95 to 280K. The experimental energy barriers (EaC2 = 0.14 eV and EaC3 = 0...... of the interstitial H2 might come from the synthesis of the compound or a side reaction with trapped synthesis residue leading to the partial oxidation of the compound and hydrogen release....

  6. The dynamics of water in hydrated white bread investigated using quasielastic neutron scattering

    International Nuclear Information System (INIS)

    Sjoestroem, J; Kargl, F; Fernandez-Alonso, F; Swenson, J

    2007-01-01

    The dynamics of water in fresh and in rehydrated white bread is studied using quasielastic neutron scattering (QENS). A diffusion constant for water in fresh bread, without temperature gradients and with the use of a non-destructive technique, is presented here for the first time. The self-diffusion constant for fresh bread is estimated to be D s = 3.8 x 10 -10 m 2 s -1 and the result agrees well with previous findings for similar systems. It is also suggested that water exhibits a faster dynamics than previously reported in the literature using equilibration of a hydration-level gradient monitored by vibrational spectroscopy. The temperature dependence of the dynamics of low hydration bread is also investigated for T = 280-350 K. The average relaxation time at constant momentum transfer (Q) shows an Arrhenius behavior in the temperature range investigated

  7. mQfit, a new program for analyzing quasi-elastic neutron scattering data

    Directory of Open Access Journals (Sweden)

    Martinez Nicolas

    2015-01-01

    Full Text Available Analysis of Quasi-elastic Neutron Scattering (QENS data of complex systems such as biological or soft matter samples in a comprehensive and explicit way often requires great efforts. Most popular software only allows to fit spectra originating from one single instrument and does not permit to extract parameters from a model that is fitted simultaneously to data taken at different instrumental resolutions. We present here a new program, mQfit (multiple QENS dataset fitting, that enables to fit QENS data taken at different spectrometers (with typical resolutions between 0.01 and 0.1 meV and momentum transfer ranges. This allows drastically reducing the number of fitting parameters. The routine is implemented with a user friendly Graphical User's Interface (GUI, and freely available. As an example, we will present results obtained on E. coli bacterial pellets, and compare them to values published in the literature.

  8. Microscopic dynamics of the hydrogen bonded systems studied by quasi-elastic slow neutron scattering

    International Nuclear Information System (INIS)

    Padureanu, I.; Aranghel, D.; Radulescu, A.; Ion, M.; Lechner, R. E.; Desmedt, A.; Pieper, J.

    2002-01-01

    provide a satisfactory description of supercooled liquid dynamics. In order to contribute to an answer, we performed a new experiment of incoherent slow neutron scattering. Part of the obtained results is presented in a previously paper. Neutron scattering experiments were done at the time of flight spectrometer NEAT of the Berlin Neutron Scattering Center(BENSC). In this study we have used cold neutrons with the wavelength of λ = 5.1 A, which corresponds to an incident energy E o = 3.145 meV and a resolution ΔE = 98 μeV (full width at half-maximum, FWHM, of the elastic line of the vanadium sample). The scattering spectra were taken with 140 detectors in a large angular range 15.41 angle -1 for the elastic wave and the energy transfer hω s (θ,ω). The final data are obtained at 27 scattering angles as a function of the energy transfer hω for 8 temperatures 50 K, 100 K, 150 K, 188 K, 240 K, 290 K, 320 K and 400 K. The data have been also analyzed in terms of the generalized frequency distribution g (ω), the angular distribution dσ/dΩ of the quasi-elastically scattered neutrons and the observed line width ΔE = f (Q 0 2 , T). An obvious feature attribute to as boson peak is present at all temperatures from 50 K to 290 K in the dynamic scattering function Ss (θ,ω) and the generalized frequency distribution g (ω)/ω 2 of glycerol. The temperature dependence of the peak position shows an anomalous behavior near T g . This effect proves a soft dynamics additionally to the acoustic modes. At the same time the temperature dependence of the FWHM of the quasielastic line leads to a possible two step process approach in glycerol. (authors)

  9. Mode coupling analysis of coherent quasi-elastic neutron scattering from fluorite-type materials approaching the superionic transition

    International Nuclear Information System (INIS)

    Chaturvedi, D.K.; Tosi, M.P.

    1987-08-01

    Neutron scattering experiments on SrCl 2 , CaF 2 and PbF 2 have shown that intensity and width of the coherent diffuse quasi-elastic spectrum increase rapidly with temperature into the fast-ion conducting phase, the main feature in the integrated quasi-elastic intensity being a peak just beyond the (200) point along the (100) direction in scattering wave vector space. The Zwanzig-Mori memory function formalism is used in this work to analyze the quasi-elastic scattering cross section from charge density fluctuations in terms of anharmonic couplings between the vibrational modes of the crystal. The two- and three-mode channels are examined for compatibility with the quasi-elastic neutron scattering evidence, on the basis of (i) energy and momentum conservation and van Hove singularity arguments and (ii) measured phonon dispersion curves along the main symmetry directions in SrCl 2 , CaF 2 , SrF 2 and BaF 2 . The analysis identifies a specific microscopic role for the Raman-active optic branches. The eigenvectors of the relevant Raman-active and partner modes in the three-mode channel describe relative displacements of the two halogens in the unit cell superposed on relative displacements of the halogen and alkaline earth components. This microscopic picture is thus consistent with the superionic transition being associated with the onset of dynamic disorder in the anionic component of the crystal. (author). 13 refs, 2 tabs

  10. Dynamics of water and ions in clays of type montmorillonite by microscopic simulation and quasi-elastic neutron scattering

    International Nuclear Information System (INIS)

    Malikova, N.

    2005-09-01

    Montmorillonite clays in low hydration states, with Na + and Cs + compensating counter ions, are investigated by a combination of microscopic simulation and quasi-elastic neutron scattering to obtain information on the local structure and dynamics of water and ions in the interlayer. At first predictions of simulation into the dynamics of water and ions at elevate temperatures are shown (0 deg C 80 deg C, pertinent for the radioactive waste disposal scenario) Marked difference is observed between the modes of diffusion of the Na + and C + counter ions. In water dynamics, a significant step towards bulk water behaviour is seen on transition from the mono- to bilayer states. Secondly, a detailed comparison between simulation and quasi-elastic neutron scattering (Neutron Spin Echo and Time-of-Flight) regarding ambient temperature water dynamics is presented. Overall, the approaches are found to be in good agreement with each other and limitations of each of the methods are clearly shown. (author)

  11. Molecular dynamics in conducting polyaniline protonated by camphor sulfonic acid as seen by quasielastic neutron scattering

    International Nuclear Information System (INIS)

    Djurado, D.; Combet, J.; Bee, M.; Rannou, P.; Dufour, B.; Pron, A.; Travers, J. P.

    2002-01-01

    Using incoherent quasielastic neutron scattering techniques, the molecular motions were investigated in fully hydrogenated and partially deuterated polyaniline protonated by camphor sulfonic acid (CSA) conducting samples. The obtained results show that on the 10 -9 -10 -12 s time scale the polymer chains do not exhibit any diffusive motions: the whole observed quasielastic scattering has accordingly to be attributed to motions of CSA ions. From our measurements two molecular movements could be differentiated. A rapid one has been attributed to the three-site rotation of methyl groups present on camphor moieties of CSA and a slower one that has been modeled as a rigid body motion of the whole CSA molecule. Due to the disordered character of the system, the methyl rotors appeared to be dynamically nonequivalent. Their dynamics was then described in terms of a log gaussian distribution of correlation times. This description allowed a good fitting of experimental data and gave an activation energy of 12.5 kJ mol-1. However, two different regimes in temperature could be distinguished. At high temperatures (T>280 K) the width of the distribution is nearly zero and thus, the methyl rotors are dynamically equivalent while it turned larger and larger when temperature is decreased below 250 K revealing that the rotors are more and more sensitive to their local environment. In the conducting samples the slowest motion clearly exists in the 280-330 K temperature range and is blocked at temperatures inferior to 250 K. This transition occurs in the temperature range in which the metal-insulator transition also happens

  12. Quasi-elastic neutron scattering studies of the slow dynamics of supercooled and glassy aspirin

    International Nuclear Information System (INIS)

    Zhang Yang; Mamontov, Eugene; Tyagi, Madhusudan; Chen, Sow-Hsin

    2012-01-01

    Aspirin, also known as acetylsalicylic acid (ASA), is not only a wonderful drug, but also a good glass former. Therefore, it serves as an important molecular system to study the near-arrest and arrested phenomena. In this paper, a high-resolution quasi-elastic neutron scattering (QENS) technique is used to investigate the slow dynamics of supercooled liquid and glassy aspirin from 410 down to 350 K. The measured QENS spectra can be analyzed with a stretched exponential model. We find that (i) the stretched exponent β(Q) is independent of the wavevector transfer Q in the measured Q range and (ii) the structural relaxation time τ(Q) follows a power-law dependence on Q. Consequently, the Q-independent structural relaxation time τ 0 can be extracted for each temperature to characterize the slow dynamics of aspirin. The temperature dependence of τ 0 can be fitted with the mode-coupling power law, the Vogel-Fulcher-Tammann equation and a universal equation for fragile glass forming liquids recently proposed by Tokuyama in the measured temperature range. The calculated dynamic response function χ T (Q, t) using the experimentally determined self-intermediate scattering function of the hydrogen atoms of aspirin shows direct evidence of the enhanced dynamic fluctuations as the aspirin is increasingly supercooled, in agreement with the fixed-time mean squared displacement (x 2 ) and the non-Gaussian parameter α 2 extracted from the elastic scattering.

  13. Quasi-Elastic Neutron Scattering Studies of the Slow Dynamics of Supercooled and Glassy Aspirin

    Energy Technology Data Exchange (ETDEWEB)

    Zhang, Yang [ORNL; Tyagi, M. [NCNR and University of Maryland; Mamontov, Eugene [ORNL; Chen, Sow-hsin H [ORNL

    2011-01-01

    Aspirin, also known as acetylsalicylic acid (ASA), is not only a wonderful drug, but also a good glass former. Therefore, it serves as an important molecular system to study the near-arrest and arrested phenomena. In this paper, a high-resolution quasi-elastic neutron scattering (QENS) technique is used to investigate the slow dynamics of supercooled liquid and glassy aspirin from 410 K down to 350 K. The measured QENS spectra can be analyzed with a stretched exponential model. We find that (i) the stretched exponent (Q) is independent of the wave vector transfer Q in the measured Q-range, and (ii) the structural relaxation time (Q) follows a power law dependence on Q. Consequently, the Q-independent structural relaxation time 0 can be extracted for each temperature to characterize the slow dynamics of aspirin. The temperature dependence of 0 can be fitted with the mode coupling power law, the Vogel-Fulcher-Tammann equation and a universal equation for fragile glass forming liquids recently proposed by M. Tokuyama in the measured temperature range. The calculated dynamic response function T(Q,t) using the experimentally determined self-intermediate scattering function of the hydrogen atoms of aspirin shows a direct evidence of the enhanced dynamic fluctuations as the aspirin is increasingly supercooled, in agreement with the fixed-time mean squared displacement x2 and non-Gaussian parameter 2 extracted from the elastic scattering.

  14. Quasielastic neutron scattering study of large amplitude motions in molecular systems

    International Nuclear Information System (INIS)

    Bee, M.

    1996-01-01

    This lecture aims at giving some illustrations of the use of Incoherent Quasielastic Neutron Scattering in the investigation of motions of atoms or molecules in phases with dynamical disorder. The general incoherent scattering function is first recalled. Then the Elastic Incoherent Structure Factor is introduced. It is shown how its determination permits to deduce a particular dynamical model. Long-range translational diffusion is illustrated by some experiments carried out with liquids or with different chemical species intercalated in porous media. Examples of rotational motions are provided by solid phases where an orientational disorder of the molecules exists. The jump model is the most commonly used and yields simple scattering laws which can be easily handled. Highly disordered crystals require a description in terms of the isotropic rotational diffusion model. Many of the present studies are concerned with rather complicated systems. Considerable help is obtained either by using selectively deuterated samples or by carrying out measurements with semi-oriented samples. (author) 5 figs., 14 refs

  15. Quasi-elastic neutron scattering studies of the slow dynamics of supercooled and glassy aspirin

    Science.gov (United States)

    Zhang, Yang; Tyagi, Madhusudan; Mamontov, Eugene; Chen, Sow-Hsin

    2012-02-01

    Aspirin, also known as acetylsalicylic acid (ASA), is not only a wonderful drug, but also a good glass former. Therefore, it serves as an important molecular system to study the near-arrest and arrested phenomena. In this paper, a high-resolution quasi-elastic neutron scattering (QENS) technique is used to investigate the slow dynamics of supercooled liquid and glassy aspirin from 410 down to 350 K. The measured QENS spectra can be analyzed with a stretched exponential model. We find that (i) the stretched exponent β(Q) is independent of the wavevector transfer Q in the measured Q range and (ii) the structural relaxation time τ(Q) follows a power-law dependence on Q. Consequently, the Q-independent structural relaxation time τ0 can be extracted for each temperature to characterize the slow dynamics of aspirin. The temperature dependence of τ0 can be fitted with the mode-coupling power law, the Vogel-Fulcher-Tammann equation and a universal equation for fragile glass forming liquids recently proposed by Tokuyama in the measured temperature range. The calculated dynamic response function χT(Q, t) using the experimentally determined self-intermediate scattering function of the hydrogen atoms of aspirin shows direct evidence of the enhanced dynamic fluctuations as the aspirin is increasingly supercooled, in agreement with the fixed-time mean squared displacement langx2rang and the non-Gaussian parameter α2 extracted from the elastic scattering.

  16. Neutron quasi-elastic scattering study of translational motions in the smectic H, C and A phases of TBBA

    International Nuclear Information System (INIS)

    Dianoux, A.J.; Volino, F.; Heidemann, A.; Hervet, H.

    1975-01-01

    Neutron quasi-elastic scattering experiments in the smectic H, C and A phases of TBBA are presented, using the high resolution backscattering technique. The data are analyzed in terms of translational motion and are characterized by an apparent self diffusion coefficient Dsub(ap). The physical meaning of Dsub(ap) is discussed in terms of the true bulk self diffusion tensor and other kinds of translational motions [fr

  17. Application of quasi-elastic neutron scattering to dynamics study of confined water

    International Nuclear Information System (INIS)

    Li Hua; Zhang Lili; Yi Zhou

    2014-01-01

    Background: Quasi-elastic neutron scattering (QENS) is an important experiment for dynamics study of confined water. It is significant to study the dynamics of confined water in cement paste. Purpose: In this paper, we have two aims. One is to present a reviewer of QENS study on dynamics of confined water in cement paste in recent years. The other is to illustrate the QENS application to the study on dynamics of confined water based on cement paste. Method: Relaxing cage model (RCM) is specially introduced for the analyses of QENS spectra. Results: Based on RCM, several parameters for describing the dynamics of confined water in cement paste, can be obtained from the analyses of QENS spectra: a fraction of mobile 'glassy' water molecules embedded in amorphous gel region surrounding the hydration products, 1-p, the capture time of confined water molecule in some place-τ 0 , the average translational relaxation time-<τ>, the self-diffusion coefficient-D, and a phenomenological shape parameter describing the uniform of amorphous in cement paste-β. Conclusion: All these provide a practical method for QENS study on dynamics of confined water in cement paste. (authors)

  18. Quasielastic scattering of slow-neutron in water-alcohol solutions

    Directory of Open Access Journals (Sweden)

    N. O. Atamas

    2010-06-01

    Full Text Available Research of molecules dynamics of solutions “water - propyl alcohol” of different concentration at the temperature 281 K is conducted by the method of slow-neutron quasi-elastic scattering. There were experimentally exposed the feature of effective self-diffusion coefficient of molecules of the indicated solutions. Based on the time- scale hierarchy the division of selfdiffusion coefficient to one-particle and collective contributions was conducted, and the time of the molecules settled life in position of equilibrium was calculated. There were also exposed the feature of self-diffusion concentration dependence of coefficient of self-diffusion and his selfpart contribution, namely: presence of two minimums is in the areas of concentrations (0,04 ÷ 0,05 of mass fraction and (0,18 ÷ 0,22 m.c. of the alcohol and continuous character of diffusion at concentrations higher then 0,4 m.c. of the alcohol. It is shown that the indicated concentration areas correspond the certain local structures of investigational solution.

  19. Analysis of quasielastic neutron scattering (QENS) data of discotic systems using different molecular dynamics (MD) models

    International Nuclear Information System (INIS)

    Kruglova, O.; Mulder, F.M.; Picken, S.J.; Stride, J.; Kearley, G.J.

    2004-01-01

    Discotic molecules are composed of an aromatic core surrounded by aliphatic chains. These molecules are of importance because they can form columns in which the π orbitals of neighbouring molecules overlap leading to conductivity along the column. These materials find applications in molecular electronics and recently--with record quantum efficiencies--in photo voltaics. Because the correlation time of the electron (or hole) hopping is in the picosecond region, molecular dynamics on this timescale is of central importance. We have recently shown that these dynamics, which is easily measured by quasielastic neutron scattering (QENS), can be understood with a rather simple 'short single-column' model via an MD simulation that reproduces the measured QENS spectra. Before progressing to the larger technologically important systems we must understand any fortuitous error cancellations that may cause the simple model to reproduce the experimental signal so well. By taking a very simple discotic, hexamethyltriphenylene (HMT), we are able to compare QENS data with three types of models: simple column, cluster and periodic. It transpires that the cluster model cannot properly accommodate inter column interactions, and a fairly modest periodic model overcomes this problem and the tendency for un-physical harmonic modes along the column

  20. Segmental dynamics in polymer melts by relaxation techniques and quasielastic neutron scattering

    Science.gov (United States)

    Colmenero, J.

    1993-01-01

    The dynamics of the segmental α-relaxation in three different polymeric systems, poly(vinyl methy ether) (PVME), poly(vinyl chloride) (PVC) and poly(bisphenol A, 2-hydroxypropylether) (PH) has been studied by means of relaxation techniques and quasielastic neutron scattering (backscattering spectrometers IN10 and IN13 at the ILL-Grenoble). By using these techniques we have covered a wide timescale ranging from mesoscopic to macroscopic times (10-10-101s). For analyzing the experimental data we have developed a phenomenological procedure in the frequency domain based on the Havriliak-Negami relaxation function which in fact implies a Kohlrausch-Williams-Watts relaxation function in the time domain. The results obtained indicate that the dynamics of the α-relaxation in a wide timescale shows a clear non-Debye behaviour. The shape of the relaxation function is found to be similar for the different techniques used and independent of temperature and momentum transfer (Q). Moreover the characteristic relaxation times deduced from the fitting of the experimental data can also be described using only one Vogel-Fulcher functional form. Besides we found that the Q-dependence of the relaxation times obtained by QENS is given by a power law, τ(Q) propto Q-n (n > 2) n being dependent on the system, and that the Q-behaviour and the non-Debye behaviour are directly correlated. We discuss this correlation taking into account several data of the dynamics of the α-relaxation previously reported in the literature. We also outline a possible scenario for explaining this empirical correlation.

  1. Dynamical Behavior of Human α-Synuclein Studied by Quasielastic Neutron Scattering.

    Directory of Open Access Journals (Sweden)

    Satoru Fujiwara

    Full Text Available α-synuclein (αSyn is a protein consisting of 140 amino acid residues and is abundant in the presynaptic nerve terminals in the brain. Although its precise function is unknown, the filamentous aggregates (amyloid fibrils of αSyn have been shown to be involved in the pathogenesis of Parkinson's disease, which is a progressive neurodegenerative disorder. To understand the pathogenesis mechanism of this disease, the mechanism of the amyloid fibril formation of αSyn must be elucidated. Purified αSyn from bacterial expression is monomeric but intrinsically disordered in solution and forms amyloid fibrils under various conditions. As a first step toward elucidating the mechanism of the fibril formation of αSyn, we investigated dynamical behavior of the purified αSyn in the monomeric state and the fibril state using quasielastic neutron scattering (QENS. We prepared the solution sample of 9.5 mg/ml purified αSyn, and that of 46 mg/ml αSyn in the fibril state, both at pD 7.4 in D2O. The QENS experiments on these samples were performed using the near-backscattering spectrometer, BL02 (DNA, at the Materials and Life Science Facility at the Japan Accelerator Research Complex, Japan. Analysis of the QENS spectra obtained shows that diffusive global motions are observed in the monomeric state but largely suppressed in the fibril state. However, the amplitude of the side chain motion is shown to be larger in the fibril state than in the monomeric state. This implies that significant solvent space exists within the fibrils, which is attributed to the αSyn molecules within the fibrils having a distribution of conformations. The larger amplitude of the side chain motion in the fibril state than in the monomeric state implies that the fibril state is entropically favorable.

  2. Dynamics of Phenanthrenequinone on Carbon Nano-Onion Surfaces Probed by Quasielastic Neutron Scattering

    International Nuclear Information System (INIS)

    Mamontov, Eugene; Brown, Gilbert M.; Overbury, Steven H.; Mavila Chathoth, Suresh

    2012-01-01

    We used quasielastic neutron scattering (QENS) to study the dynamics of phenanthrenequinone (PQ) on the surface of onion-like carbon (OLC), or so called carbon onions, as a function of surface coverage and temperature. For both the high- and low-coverage samples, we observed two diffusion processes; a faster process and nearly an order of magnitude slower process. On the high-coverage surface, the slow diffusion process is of long-range translational character, whereas the fast diffusion process is spatially localized on the length scale of ∼ 4.7. On the low-coverage surface, both diffusion processes are spatially localized; on the same length scale of ∼ 4.7 for the fast diffusion and a somewhat larger length scale for the slow diffusion. Arrhenius temperature dependence is observed except for the long-range diffusion on the high-coverage surface. We attribute the fast diffusion process to the generic localized in-cage dynamics of PQ molecules, and the slow diffusion process to the long-range translational dynamics of PQ molecules, which, depending on the coverage, may be either spatially restricted, or long-range. On the low-coverage surface, uniform surface coverage is not attained, and the PQ molecules experience the effect of spatial constraints on their long-range translational dynamics. Unexpectedly, the dynamics of PQ molecules on OLC as a function of temperature and surface coverage bears qualitative resemblance to the dynamics of water molecules on oxide surfaces, including practically temperature-independent residence times for the low-coverage surface. The dynamics features that we observed may be universal across different classes of surface adsorbates.

  3. Static and quasi-elastic small angle neutron scattering on biocompatible ionic ferrofluids: magnetic and hydrodynamic interactions

    CERN Document Server

    Gazeau, F; Dubois, E; Perzynski, R

    2003-01-01

    We investigate the structure and dynamics of ionic magnetic fluids (MFs), based on ferrite nanoparticles, dispersed at pH approx 7 either in H sub 2 O or in D sub 2 O. Polarized and non-polarized static small angle neutron scattering (SANS) experiments in zero magnetic field allow us to study both the magnetic and the nuclear contributions to the neutron scattering. The magnetic interparticle attraction is probed separately from the global thermodynamic repulsion and compares well to direct magnetic susceptibility measurements. The magnetic interparticle correlation is in these fluid samples independent of the probed spatial scale. In contrast, a spatial dependence of the interparticle correlation is evidenced at large PHI by the nuclear structure factor. A model of magnetic interaction quantitatively explains the under-field anisotropy of the SANS nuclear contribution. In a quasi-elastic neutron spin-echo experiment, we probe the Brownian dynamics of translation of the nanoparticles in the range 1.3 sup<=...

  4. Intramolecular diffusive motion in alkane monolayers studied by high-resolution quasielastic neutron scattering and molecular dynamics simulations

    DEFF Research Database (Denmark)

    Hansen, Flemming Yssing; Criswell, L.; Fuhrmann, D

    2004-01-01

    Molecular dynamics simulations of a tetracosane (n-C24H50) monolayer adsorbed on a graphite basal-plane surface show that there are diffusive motions associated with the creation and annihilation of gauche defects occurring on a time scale of similar to0.1-4 ns. We present evidence...... that these relatively slow motions are observable by high-energy-resolution quasielastic neutron scattering (QNS) thus demonstrating QNS as a technique, complementary to nuclear magnetic resonance, for studying conformational dynamics on a nanosecond time scale in molecular monolayers....

  5. Hydrogen dynamics in Na3AlH6: A combined density functional theory and quasielastic neutron scattering study

    DEFF Research Database (Denmark)

    Voss, Johannes; Shi, Qing; Jacobsen, Hjalte Sylvest

    2007-01-01

    alanate with TiCl3, and here we study hydrogen dynamics in doped and undoped Na3AlH6 using a combination of density functional theory calculations and quasielastic neutron scattering. The hydrogen dynamics is found to be vacancy mediated and dominated by localized jump events, whereas long-range bulk......Understanding the elusive catalytic role of titanium-based additives on the reversible hydrogenation of complex hydrides is an essential step toward developing hydrogen storage materials for the transport sector. Improved bulk diffusion of hydrogen is one of the proposed effects of doping sodium...... defect motion in sodium alanate could result from vacancy-mediated sodium diffusion....

  6. Point defect dynamics in sodium aluminum hydrides - a combined quasielastic neutron scattering and density functional theory study

    DEFF Research Database (Denmark)

    Shi, Qing; Voss, Johannes; Jacobsen, H.S.

    2007-01-01

    we study hydrogen dynamics in undoped and TiCl3-doped samples of NaAlH4 and Na3AlH6 using a combination of density functional theory calculations and quasielastic neutron scattering. Hydrogen dynamics is found to be limited and mediated by hydrogen vacancies in both alanate phases, requiring......Understanding the catalytic role of titanium-based additives on the reversible hydrogenation of complex metal hydrides is an essential step towards developing hydrogen storage materials for the transport sector. Improved bulk diffusion of hydrogen is one of the proposed catalytic effects, and here...

  7. Quasielastic neutron scattering measurements and ab initio MD-simulations on single ion motions in molten NaF

    Energy Technology Data Exchange (ETDEWEB)

    Demmel, F. [ISIS Facility, Rutherford Appleton Laboratory, Didcot OX11 0QX (United Kingdom); Mukhopadhyay, S. [ISIS Facility, Rutherford Appleton Laboratory, Didcot OX11 0QX (United Kingdom); Department of Materials, Imperial College London, Exhibition Road, London SW7 2AZ (United Kingdom)

    2016-01-07

    The ionic stochastic motions in the molten alkali halide NaF are investigated by quasielastic neutron scattering and first principles molecular dynamics simulation. Quasielastic neutron scattering was employed to extract the diffusion behavior of the sodium ions in the melt. An extensive first principles based simulation on a box of up to 512 particles has been performed to complement the experimental data. From that large box, a smaller 64-particle box has then been simulated over a runtime of 60 ps. A good agreement between calculated and neutron data on the level of spectral shape has been obtained. The obtained sodium diffusion coefficients agree very well. The simulation predicts a fluorine diffusion coefficient similar to the sodium one. Applying the Nernst-Einstein equation, a remarkable large cross correlation between both ions can be deduced. The velocity cross correlations demonstrate a positive correlation between the ions over a period of 0.1 ps. That strong correlation is evidence that the unlike ions do not move completely statistically independent and have a strong association over a short period of time.

  8. Structural dynamics of supercooled water from quasielastic neutron scattering and molecular simulations.

    Science.gov (United States)

    Qvist, Johan; Schober, Helmut; Halle, Bertil

    2011-04-14

    One of the outstanding challenges presented by liquid water is to understand how molecules can move on a picosecond time scale despite being incorporated in a three-dimensional network of relatively strong H-bonds. This challenge is exacerbated in the supercooled state, where the dramatic slowing down of structural dynamics is reminiscent of the, equally poorly understood, generic behavior of liquids near the glass transition temperature. By probing single-molecule dynamics on a wide range of time and length scales, quasielastic neutron scattering (QENS) can potentially reveal the mechanistic details of water's structural dynamics, but because of interpretational ambiguities this potential has not been fully realized. To resolve these issues, we present here an extensive set of high-quality QENS data from water in the range 253-293 K and a corresponding set of molecular dynamics (MD) simulations to facilitate and validate the interpretation. Using a model-free approach, we analyze the QENS data in terms of two motional components. Based on the dynamical clustering observed in MD trajectories, we identify these components with two distinct types of structural dynamics: picosecond local (L) structural fluctuations within dynamical basins and slower interbasin jumps (J). The Q-dependence of the dominant QENS component, associated with J dynamics, can be quantitatively rationalized with a continuous-time random walk (CTRW) model with an apparent jump length that depends on low-order moments of the jump length and waiting time distributions. Using a simple coarse-graining algorithm to quantitatively identify dynamical basins, we map the newtonian MD trajectory on a CTRW trajectory, from which the jump length and waiting time distributions are computed. The jump length distribution is gaussian and the rms jump length increases from 1.5 to 1.9 Å as the temperature increases from 253 to 293 K. The rms basin radius increases from 0.71 to 0.75 Å over the same range. The

  9. Water dynamics in hardened ordinary Portland cement paste or concrete: from quasielastic neutron scattering.

    Science.gov (United States)

    Bordallo, Heloisa N; Aldridge, Laurence P; Desmedt, Arnaud

    2006-09-14

    Portland cement reacts with water to form an amorphous paste through a chemical reaction called hydration. In concrete the formation of pastes causes the mix to harden and gain strength to form a rock-like mass. Within this process lies the key to a remarkable peculiarity of concrete: it is plastic and soft when newly mixed, strong and durable when hardened. These qualities explain why one material, concrete, can build skyscrapers, bridges, sidewalks and superhighways, houses, and dams. The character of the concrete is determined by the quality of the paste. Creep and shrinkage of concrete specimens occur during the loss and gain of water from cement paste. To better understand the role of water in mature concrete, a series of quasielastic neutron scattering (QENS) experiments were carried out on cement pastes with water/cement ratio varying between 0.32 and 0.6. The samples were cured for about 28 days in sealed containers so that the initial water content would not change. These experiments were carried out with an actual sample of Portland cement rather than with the components of cement studied by other workers. The QENS spectra differentiated between three different water interactions: water that was chemically bound into the cement paste, the physically bound or "glassy water" that interacted with the surface of the gel pores in the paste, and unbound water molecules that are confined within the larger capillary pores of cement paste. The dynamics of the "glassy" and "unboud" water in an extended time scale, from a hundred picoseconds to a few nanoseconds, could be clearly differentiated from the data. While the observed motions on the picosecond time scale are mainly stochastic reorientations of the water molecules, the dynamics observed on the nanosecond range can be attributed to long-range diffusion. Diffusive motion was characterized by diffusion constants in the range of (0.6-2) 10(-9) m(2)/s, with significant reduction compared to the rate of diffusion

  10. Rotation of methyl side groups in polymers: A Fourier transform approach to quasielastic neutron scattering. 1: Homopolymers

    International Nuclear Information System (INIS)

    Arrighi, V.; Higgins, J.S.; Howells, W.S.

    1995-01-01

    The rotational motion of the ester methyl group in poly(methyl methacrylate) (PMMA) was investigated using quasielastic neutron scattering (QENS). A comparison between the authors results and the QENS data reported in the literature for PMMA-d 5 indicates that the amount of quasielastic broadening is highly dependent upon the energy resolution of the spectrometer. This anomalous behavior is here attributed to the method of analysis, namely, the use of a single rotational frequency. Such a procedure leads to a non-Arrhenius temperature dependence, to a temperature-dependent elastic incoherent structure factor, and to values of rotational frequency which are resolution dependent. They propose an alternative approach to the analysis of the QENS data which accounts for the existence of a distribution of rotational frequencies. The frequency data are Fourier transformed to the time domain, and the intermediate scattering function is fitted using a stretched exponential or Kohlraush-Williams-Watts function. The excellent overlap between data from different spectrometers leaves no doubt on the adequacy of their procedure. Measurements of the ether methyl group rotation in poly(vinyl methyl ether) (PVME) are also reported. The PVME data confirm that the behavior observed for PMMA-d 5 is likely to be a common feature to all polymeric systems

  11. Small angle, quasielastic and inelastic neutron scattering from 0.85AgPO3-0.15PbI2 glass

    International Nuclear Information System (INIS)

    Malugani, J.P.; Tachez, M.; Mercier, R.

    1987-01-01

    A small angle neutron scattering (SANS) experiment and a quasielastic neutron scattering (QENS) experiment were performed on the fast ionic conductor 0.85AgPO 3 -0.15PbI 2 , which is a vitreous electrolyte. The SANS data show that the scattering obeys Guinier's law for Q -2 A; dispersed heterogeneities are present in the glass with a mean radius of gyration of 20 A. The QENS spectra show a quasielastic broadening of the elastic peak and a long tail up to 40 meV which is due to an inelastic distribution. The results seem to confirm the hypothesis on the structure of this glass: small 'clusters' of AgI with tetrahedral coordination are dispersed in the AgPO 3 host glass. In order to build these clusters, an exchange between Ag + and Pb 2+ is proposed. 18 refs.; 6 figs.; 2 tabs

  12. Hydrogen dynamics in the low temperature phase of LiBH{sub 4} probed by quasielastic neutron scattering

    Energy Technology Data Exchange (ETDEWEB)

    Remhof, Arndt, E-mail: arndt.remhof@empa.ch [Empa, Swiss Federal Institute for Materials Science and Technology, Hydrogen and Energy, CH-8600 Dübendorf (Switzerland); Züttel, Andreas [Empa, Swiss Federal Institute for Materials Science and Technology, Hydrogen and Energy, CH-8600 Dübendorf (Switzerland); Ramirez-Cuesta, Timmy; García-Sakai, Victoria [ISIS Facility, Rutherford Appleton Laboratory, Chilton, Didcot, Oxon OX11 0QX (United Kingdom); Frick, Bernhard [Institut Laue-Langevin, F-38002 Grenoble (France)

    2013-12-12

    Highlights: • Inelastic fixed window sans offer new possibilities in neutron backscattering spectrometers. • Two different kind of reorientational motion were identified in the low temperature phase of LiBH{sub 4}. • Thermally activated jump rotation. - Abstract: LiBH{sub 4} contains 18.5 wt% hydrogen and undergoes a structural phase transition (orthorhombic → hexagonal) at 381 K which is associated with a large increase in hydrogen and lithium solid-state mobility. We investigated the hydrogen dynamics in the low temperature phase of LiBH{sub 4} by quasielastic neutron scattering, including a new kind of inelastic fixed window scan (IFWS). In the temperature range from 175 to 380 K the H-dynamics is dominated by thermally activated rotational jumps of the [BH{sub 4}]{sup −} anion around the c3 axis with an activation energy of about 162 meV. In agreement with earlier NMR data, a second type of thermally activated motion with an activation energy of about 232 meV could be identified using the IFWS. The present study of hydrogen dynamics in LiBH{sub 4} illustrates the feasibility of using IFWS on neutron backscattering spectrometers as a probe of localised motion.

  13. Quasi-elastic scattering

    International Nuclear Information System (INIS)

    Pizzi, J.R.

    1975-01-01

    In a first part, the kinematical conditions which are chosen to study quasi free scattering reactions are presented, as well as the impulse approximation which is used to interpret the experimental data. Then, the evolution of the study of these reactions in the last few years is analyzed. Three recent experiments are presented and discussed. Two of them deal with α-clusters studied by (p,pα) reaction at 157 and 600MeV. The third is concerned with d, t and 3 He clusters studied by (p,px) reaction at 75MeV [fr

  14. Quasi-elastic neutron scattering study of a re-entrant side-chain liquid-crystal polyacrylate

    Science.gov (United States)

    Benguigui, L.; Noirez, L.; Kahn, R.; Keller, P.; Lambert, M.; Cohen de Lara, E.

    1991-04-01

    We present a first investigation of the dynamics of a side chain liquid crystal polyacrylate in the isotropic (I), nematic (N), smectic A (SA), and re-entrant nematic (NRe) phases by means of quasi-elastic neutron scattering. The motion or/and the mobility of the mesogen protons decreases as soon as the temperature decreases after the isotropic-nematic transition. The I-N and SA-NRe transitions corrspond to a jump in the curve of the Elastic Incoherent Structure Factor (ratio: elastic scattering/ total scattering) versus temperature, on the other hand the transition N-SA occurs without any change of slope. We conclude that the local order is very similar in the nematic and the smectic A phases. Nous présentons une première étude dynamique par diffusion quasi-élastique des neutrons, d'un échantillon de polyacrylate mésomorphe en peigne dans chacune des phases : isotrope, nématique, smectique et nématique rentrante. On montre que le mouvement et/ou la mobilité des protons du mésogène se restreint à mesure que la température diminue après la transition isotrope-nématique. Contrairement à la transition N-SA, les transitions I-N et SA-NRe correspondent à une discontinuité dans la courbe du Facteur de Structure Incohérent Elastique (rapport : intensité élastique/intensité totale) en fonction de la température ; l'ordre local semble donc très proche pour les phases nématique et smectique.

  15. On possible contribution of standing wave like spacer dynamics in polymer liquid crystals to quasi-elastic cold neutron scattering spectra

    International Nuclear Information System (INIS)

    Jecl, R.; Cvikl, B.

    1998-01-01

    The quasi-elastic cold neutron incoherent scattering law, QNS, for the assumed case of transversal standing wave type of motion of the linear chain a spacer-of the polyacrylate polymer liquid crystal, based upon the random walk of the particle between two perfectly potential barriers, is derived. The spacer protons are taken to vibrate (within the stationary plane) transversely to the line joining the oxygen atoms in a way where they are all simultaneously displaced in the same direction with amplitudes of the standing wave fundamental mode of the vibration excited. The calculated relevant incoherent scattering law is found to be a non-distinct function of the scattering vector Q, in the sense that the postulated dynamical effect of the spacer protons causes the peak value of the calculated incoherent scattering law, S(Q,ω), to remain constant throughout the experimentally accessible range of the scattering vector Q. It appears that, when the experimental resolution broadening effects is taken into account, the contribution of the postulated dynamical behavior to the measured QNS spectra might be small, particularly so, if dome additional motion of the scatters is present, and consequently the standing wave like spacer dynamics in polymer liquid crystals will be very difficult to be identified uniquely in the quasielastic neutron scattering experiments.(author)

  16. Levitation effect in zeolites: Quasielastic neutron scattering and molecular dynamics study of pentane isomers in zeolite NaY.

    Science.gov (United States)

    Borah, Bhaskar J; Jobic, H; Yashonath, S

    2010-04-14

    We report the quasielastic neutron scattering (QENS) and molecular dynamics (MD) investigations into diffusion of pentane isomers in zeolite NaY. The molecular cross section perpendicular to the long molecular axis varies for the three isomers while the mass and the isomer-zeolite interaction remains essentially unchanged. Both QENS and MD results show that the branched isomers neopentane and isopentane have higher self-diffusivities as compared with n-pentane at 300 K in NaY zeolite. This result provides direct experimental evidence for the existence of nonmonotonic, anomalous dependence of self-diffusivity on molecular diameter known as the levitation effect. The energetic barrier at the bottleneck derived from MD simulations exists for n-pentane which lies in the linear regime while no such barrier is seen for neopentane which is located clearly in the anomalous regime. Activation energy is in the order E(a)(n-pentane)>E(a)(isopentane)>E(a)(neopentane) consistent with the predictions of the levitation effect. In the liquid phase, it is seen that D(n-pentane)>D(isopentane)>D(neopentane) and E(a)(n-pentane)scattering function for small wavenumbers obtained from MD follows a single exponential decay for neopentane and isopentane. For n-pentane, a single exponential fit provides a poor fit especially at short times. Cage residence time is largest for n-pentane and lowest for neopentane. For neopentane, the width of the self-part of the dynamic structure factor shows a near monotonic decrease with wavenumber. For n-pentane a minimum is seen near k=0.5 A(-1) suggesting a slowing down of motion around the 12-ring window, the bottleneck for diffusion. Finally, the result that the branched isomer has a higher diffusivity as compared with the linear analog is at variation from what is normally seen.

  17. Probing the hydrogen equilibrium and kinetics in zeolite imidazolate frameworks via molecular dynamics and quasi-elastic neutron scattering experiments.

    Science.gov (United States)

    Pantatosaki, Evangelia; Jobic, Hervé; Kolokolov, Daniil I; Karmakar, Shilpi; Biniwale, Rajesh; Papadopoulos, George K

    2013-01-21

    The problem of simulating processes involving equilibria and dynamics of guest sorbates within zeolitic imidazolate frameworks (ZIF) by means of molecular dynamics (MD) computer experiments is of growing importance because of the promising role of ZIFs as molecular "traps" for clean energy applications. A key issue for validating such an atomistic modeling attempt is the possibility of comparing the MD results, with real experiments being able to capture analogous space and time scales to the ones pertained to the computer experiments. In the present study, this prerequisite is fulfilled through the quasi-elastic neutron scattering technique (QENS) for measuring self-diffusivity, by elaborating the incoherent scattering signal of hydrogen nuclei. QENS and MD experiments were performed in parallel to probe the hydrogen motion, for the first time in ZIF members. The predicted and measured dynamics behaviors show considerable concentration variation of the hydrogen self-diffusion coefficient in the two topologically different ZIF pore networks of this study, the ZIF-3 and ZIF-8. Modeling options such as the flexibility of the entire matrix versus a rigid framework version, the mobility of the imidazolate ligand, and the inclusion of quantum mechanical effects in the potential functions were examined in detail for the sorption thermodynamics and kinetics of hydrogen and also of deuterium, by employing MD combined with Widom averaging towards studying phase equilibria. The latter methodology ensures a rigorous and efficient way for post-processing the dynamics trajectory, thereby avoiding stochastic moves via Monte Carlo simulation, over the large number of configurational degrees of freedom a nonrigid framework encompasses.

  18. A new apparatus design for high temperature (up to 950 °C) quasi-elastic neutron scattering in a controlled gaseous environment

    International Nuclear Information System (INIS)

    Al-Wahish, Amal; Armitage, D.; Hill, B.; Mills, R.; Santodonato, L.; Herwig, K. W.; Al-Binni, U.; Jalarvo, N.; Mandrus, D.

    2015-01-01

    A design for a sample cell system suitable for high temperature Quasi-Elastic Neutron Scattering (QENS) experiments is presented. The apparatus was developed at the Spallation Neutron Source in Oak Ridge National Lab where it is currently in use. The design provides a special sample cell environment under controlled humid or dry gas flow over a wide range of temperature up to 950 °C. Using such a cell, chemical, dynamical, and physical changes can be studied in situ under various operating conditions. While the cell combined with portable automated gas environment system is especially useful for in situ studies of microscopic dynamics under operational conditions that are similar to those of solid oxide fuel cells, it can additionally be used to study a wide variety of materials, such as high temperature proton conductors. The cell can also be used in many different neutron experiments when a suitable sample holder material is selected. The sample cell system has recently been used to reveal fast dynamic processes in quasi-elastic neutron scattering experiments, which standard probes (such as electrochemical impedance spectroscopy) could not detect. In this work, we outline the design of the sample cell system and present results demonstrating its abilities in high temperature QENS experiments

  19. A new apparatus design for high temperature (up to 950°C) quasi-elastic neutron scattering in a controlled gaseous environment.

    Science.gov (United States)

    al-Wahish, Amal; Armitage, D; al-Binni, U; Hill, B; Mills, R; Jalarvo, N; Santodonato, L; Herwig, K W; Mandrus, D

    2015-09-01

    A design for a sample cell system suitable for high temperature Quasi-Elastic Neutron Scattering (QENS) experiments is presented. The apparatus was developed at the Spallation Neutron Source in Oak Ridge National Lab where it is currently in use. The design provides a special sample cell environment under controlled humid or dry gas flow over a wide range of temperature up to 950 °C. Using such a cell, chemical, dynamical, and physical changes can be studied in situ under various operating conditions. While the cell combined with portable automated gas environment system is especially useful for in situ studies of microscopic dynamics under operational conditions that are similar to those of solid oxide fuel cells, it can additionally be used to study a wide variety of materials, such as high temperature proton conductors. The cell can also be used in many different neutron experiments when a suitable sample holder material is selected. The sample cell system has recently been used to reveal fast dynamic processes in quasi-elastic neutron scattering experiments, which standard probes (such as electrochemical impedance spectroscopy) could not detect. In this work, we outline the design of the sample cell system and present results demonstrating its abilities in high temperature QENS experiments.

  20. Reorientations in [Mg(H2O)6](CLO4)2 studied by the proton magnetic resonance and the quasielastic neutron scattering methods

    International Nuclear Information System (INIS)

    Svare, I.; Fimland, B.O.; Janik, J.A.; Janik, J.M.; Mikuli, E.; Migdal-Mikuli, A.

    1980-01-01

    Proton magnetic relaxation measurements carried out for [Mg(H 2 O)XL6](CLO 4 ) 2 revealed two processes responsible for T 1 vs temperature dependence: one connected with H 2 O 180deg flips about the symmetry axes and second connected with a tumbling of the complex cation. Quasielastic neutron scattering measurements gave another evidence of H 2 O 180deg flips. The reorientational corelation times, which in the 273 K - 325 K region are of the order of picoseconds, as derived from NMR coincide perfectly well with those derived from QNS. (author)

  1. Hydrogen dynamics in Na3AlH6: A combined density functional theory and quasielastic neutron scattering study

    DEFF Research Database (Denmark)

    Zsigmond, G.; Manoshin, S.; Lieutenant, K.

    2007-01-01

    Handling of polarization became very important in simulations of neutron scattering. One of the very comprehensive and open-source neutron simulation package, VITESS, has been intensely involved in polarized neutron simulations. Several examples will be shown here. Another similar package NISP also...... contains polarization tools. McStas has implemented an initial set of routines handling polarization, as our examples will also show....

  2. Self-motion and the α-relaxation in glass-forming polymers. Molecular dynamic simulation and quasielastic neutron scattering results in polyisoprene

    International Nuclear Information System (INIS)

    Colmenero, Juan; Arbe, Arantxa; Alvarez, Fernando; Monkenbusch, Michael; Richter, Dieter; Farago, Bela; Frick, Bernhard

    2003-01-01

    The momentum transfer dependence of the self-motion of main chain hydrogens in the α-relaxation regime of a glass forming polymer, polyisoprene, has been thoroughly investigated by a combined effort involving fully atomistic molecular dynamic simulations and quasielastic neutron scattering measurements. In this way, we have established the existence of a crossover from a Gaussian regime of sublinear diffusion to a strongly non-Gaussian regime at short distances. We show that an anomalous jump diffusion model with a distribution of jump lengths gives rise to such a crossover. This model leads to a time-dependent non-Gaussian parameter exhibiting all features revealed so far from various simulations of different glass forming systems

  3. Quasielastic neutron scattering and infra-red band contour study of H2O reorientations in [Ni(H2O)6] (ClO4)2

    International Nuclear Information System (INIS)

    Janik, J.A.; Janik, J.M.; Otnes, K.; Stanek, T.

    1980-01-01

    IR band contour measurements carried out for [Ni(H 2 O) 6 ] (ClO 4 ) 2 revealed an existence of fast H 2 O 180 deg flips around Ni-O axes at room temperatures. These flips were subjected to a more accurate study by the quasielastic neutron scattering method. Correlation times of the order of picosecond were obtained for room temperatures and the barrier to rotation of ca. 7 kcal/mole. The results are compared to those previously obtained for [Mg(H 2 O) 6 ] (ClO 4 ) 2 and also to those for [Ni(NH 3 ) 6 ] (ClO 4 ) 2 and [Mg(NH 3 ) 6 ] (ClO 4 ) 2 . (author)

  4. New Insights into the Molecular Dynamics of P3HT:PCBM Bulk Heterojunction: A Time-of-Flight Quasi-Elastic Neutron Scattering Study.

    Science.gov (United States)

    Guilbert, Anne A Y; Zbiri, Mohamed; Jenart, Maud V C; Nielsen, Christian B; Nelson, Jenny

    2016-06-16

    The molecular dynamics of organic semiconductor blend layers are likely to affect the optoelectronic properties and the performance of devices such as solar cells. We study the dynamics (5-50 ps) of the poly(3-hexylthiophene) (P3HT): phenyl-C61-butyric acid methyl ester (PCBM) blend by time-of-flight quasi-elastic neutron scattering, at temperatures in the range 250-360 K, thus spanning the glass transition temperature region of the polymer and the operation temperature of an OPV device. The behavior of the QENS signal provides evidence for the vitrification of P3HT upon blending, especially above the glass transition temperature, and the plasticization of PCBM by P3HT, both dynamics occurring on the picosecond time scale.

  5. Elastic scattering and quasi-elastic transfers

    International Nuclear Information System (INIS)

    Mermaz, M.C.

    1978-01-01

    Experiments are presented which it will be possible to carry out at GANIL on the elastic scattering of heavy ions: diffraction phenomena if the absorption is great, refraction phenomena if absorption is low. The determination of the optical parameters can be performed. The study of the quasi-elastic transfer reactions will make it possible to know the dynamics of the nuclear reactions, form exotic nuclei and study their energy excitation spectrum, and analyse the scattering and reaction cross sections [fr

  6. Quasielastic electron scattering from 40Ca

    International Nuclear Information System (INIS)

    Williamson, C.F.; Yates, T.C.; Schmitt, W.M.; Osborn, M.; Deady, M.; Zimmerman, P.D.; Blatchley, C.C.; Seth, K.K.; Sarmiento, M.; Parker, B.; Jin, Y.; Wright, L.E.; Onley, D.S.

    1997-01-01

    Differential cross sections for quasielastic electron scattering on 40 Ca have been measured at laboratory scattering angles of 45.5 degree, 90 degree, and 140 degree with bombarding energies ranging from 130 to 840 MeV. Transverse and longitudinal response functions have been extracted for momentum transfers from 300 to 500 MeV/c. Contrary to some previously reported results, the total observed longitudinal strength agrees with the relativistic Fermi gas prediction to within ±18%. copyright 1997 The American Physical Society

  7. First measurement of the electric formfactor of the neutron in the exclusive quasielastic scattering of polarized electrons from polarized 3He

    International Nuclear Information System (INIS)

    Meyerhoff, M.; Eyl, D.; Frey, A.; Andresen, H.G.; Annand, J.R.M.; Aulenbacher, K.; Becker, J.; Blume-Werry, J.; Dombo, T.; Drescher, P.; Ducret, J.E.; Fischer, H.; Grabmayr, P.; Hall, S.; Hartmann, P.; Hehl, T.; Heil, W.; Hoffmann, J.; Kellie, J.D.; Klein, F.; Leduc, M.; Moeller, H.; Nachtigall, C.; Ostrick, M.; Otten, E.W.; Owens, R.O.; Pluetzer, S.; Reichert, E.; Rohe, D.; Schaefer, M.; Schearer, L.D.; Schmieden, H.; Steffens, K.; Surkau, R.; Walcher, T.

    1995-01-01

    A first measurement of the asymmetry in quasielastic scattering of longitudinally polarized electrons from a polarized 3 He gas target in coincidence with the knocked out neutron is reported. This measurement was made feasible by the cw beam of the 855 meV Mainz Microtron MAMI. It allows a determination of the electric formfactor of the neutron G n E independent of binding effects to first order. At bar Q 2 =0.31 (GeV/c) 2 two asymmetries bar A parallel (rvec S He parallel rvec q) and bar A perpendicular (rvec S He perpendicular rvec q) have been measured giving bar A parallel =(-7.40±0.73%) and bar A perpendicular =(0.89±0.30)%. The ratio bar A perpendicular /bar A parallel is independent of the absolute value of the electron and target polarization and yields G n E =0.035±0.012±0.005. copyright 1995 American Institute of Physics

  8. Hydrophobic hydration and anomalous excess partial molar volume of tert-butyl alcohol-water mixture studied by quasielastic neutron scattering

    International Nuclear Information System (INIS)

    Nakada, Masaru; Maruyama, Kenji; Misawa, Masakatsu; Yamamuro, Osamu

    2007-01-01

    Quasielastic neutron scattering has been used to investigate the hydration of alcohol clusters in tert-butyl alcohol-water mixture. The measurements were made in a range of alcohol concentration, x TBA , from 0.0 to 0.17 in mole fraction at 25degC. Fraction, α, of water molecules hydrated to fractal-surface of alcohol clusters in tert-butyl alcohol-water mixture was obtained as a function of alcohol concentration. Average hydration number N WS of tert-butyl alcohol molecule was derived from the value of α as a function of alcohol concentration. The value of N WS for an isolated alcohol molecule in water was 19-21. The anomalous excess partial molar volume of tert-butyl alcohol-water mixture was interpreted successfully by applying the same model with the same values of volume parameter as used for 1-propanol-water mixture, δ 1 (=-0.36 cm 3 ·mol -1 ) and δ 2 (=0.60 cm 3 ·mol -1 ). (author)

  9. Hydration of alcohol clusters in 1-propanol-water mixture studied by quasielastic neutron scattering and an interpretation of anomalous excess partial molar volume.

    Science.gov (United States)

    Misawa, M; Inamura, Y; Hosaka, D; Yamamuro, O

    2006-08-21

    Quasielastic neutron scattering measurements have been made for 1-propanol-water mixtures in a range of alcohol concentration from 0.0 to 0.167 in mole fraction at 25 degrees C. Fraction alpha of water molecules hydrated to fractal surface of alcohol clusters in 1-propanol-water mixture was obtained as a function of alcohol concentration. Average hydration number N(ws) of 1-propanol molecule is derived from the value of alpha as a function of alcohol concentration. By extrapolating N(ws) to infinite dilution, we obtain values of 12-13 as hydration number of isolated 1-propanol molecule. A simple interpretation of structural origin of anomalous excess partial molar volume of water is proposed and as a result a simple equation for the excess partial molar volume is deduced in terms of alpha. Calculated values of the excess partial molar volumes of water and 1-propanol and the excess molar volume of the mixture are in good agreement with experimental values.

  10. Temperature and momentum transfer dependence of the dynamics of the α-relaxation in polymer melts. A quasielastic neutron scattering study

    Science.gov (United States)

    Colmenero, J.; Alegría, A.; Arbe, A.; Frick, B.

    1992-12-01

    The dynamics of the α-relaxation in three glass-forming polymeric systems, poly(vinyl methyl ether) (PVME), poly(vinyl chloride) (PVC), and poly(bisphenol A, 2-hydroxypropylether) (PH) has been studied by means of quasielastic neutron scattering and compared with the results obtained from relaxation techniques. The results indicate that the dynamics of the α-relaxation in a wide timescale shows a clear non-Debye behaviour and can be well described by means of the same spectral shape, which is found to be independent of temperature and momentum transfer ( Q). Moreover, the Havriliak-Negami characteristic times deduced from the fitting of the experimental data can also be described using only one Vogel-Fulcher functional form. This implies a self-consistent description of the dynamics of the α-relaxation obtained by very different probes. Besides, we found that the Q-dependence of the characteristic times obtained by QENS is given by a power law, τ(Q) ∝ Q - n ( n > 2), n being dependent on the system, and that the Q-behaviour and the non-Debye behaviour are directly correlated. These results have main implications about the physical mechanisms behind the dynamics of the α-relaxation.

  11. Hindered rotational energy barriers of BH4- tetrahedra in β-Mg(BH4)2 from quasielastic neutron scattering and DFT calculations

    DEFF Research Database (Denmark)

    Blanchard, Didier; Maronsson, Jon Bergmann; Riktor, M.D.

    2012-01-01

    , around the 2-fold (C2) and 3-fold (C3) axes were observed at temperatures from 120 to 440 K. The experimentally obtained activation energies (EaC2 = 39 and 76 meV and EaC3 = 214 meV) and mean residence times between reorientational jumps are comparable with the energy barriers obtained from DFT......In this work, hindered rotations of the BH4- tetrahedra in Mg(BH4)2 were studied by quasielastic neutron scattering, using two instruments with different energy resolution, in combination with density functional theory (DFT) calculations. Two thermally activated reorientations of the BH4- units...... calculations. A linear dependency of the energy barriers for rotations around the C2 axis parallel to the Mg-Mg axis with the distance between these two axes was revealed by the DFT calculations. At the lowest temperature (120 K) only 15% of the BH4- units undergo rotational motion and from comparison with DFT...

  12. Self and transport diffusivity of CO2 in the metal-organic framework MIL-47(V) explored by quasi-elastic neutron scattering experiments and molecular dynamics simulations.

    Science.gov (United States)

    Salles, Fabrice; Jobic, Hervé; Devic, Thomas; Llewellyn, Philip L; Serre, Christian; Férey, Gérard; Maurin, Guillaume

    2010-01-26

    Quasi-elastic neutron scattering measurements are combined with molecular dynamics simulations to determine the self-diffusivity, corrected diffusivity, and transport diffusivity of CO(2) in the metal-organic framework MIL-47(V) (MIL = Materials Institut Lavoisier) over a wide range of loading. The force field used for describing the host/guest interactions is first validated on the thermodynamics of the MIL-47(V)/CO(2) system, prior to being transferred to the investigations of the dynamics. A decreasing profile is then deduced for D(s) and D(o) whereas D(t) presents a non monotonous evolution with a slight decrease at low loading followed by a sharp increase at higher loading. Such decrease of D(t) which has never been evidenced in any microporous systems comes from the atypical evolution of the thermodynamic correction factor that reaches values below 1 at low loading. This implies that, due to intermolecular interactions, the CO(2) molecules in MIL-47(V) do not behave like an ideal gas. Further, molecular simulations enabled us to elucidate unambiguously a 3D diffusion mechanism within the pores of MIL-47(V).

  13. Quasi-Elastic Light Scattering in Ophthalmology

    Science.gov (United States)

    Ansari, Rafat R.

    The eye is not just a "window to the soul"; it can also be a "window to the human body." The eye is built like a camera. Light which travels from the cornea to the retina traverses through tissues that are representative of nearly every tissue type and fluid type in the human body. Therefore, it is possible to diagnose ocular and systemic diseases through the eye. Quasi-elastic light scattering (QELS) also known as dynamic light scattering (DLS) is a laboratory technique routinely used in the characterization of macromolecular dispersions. QELS instrumentation has now become more compact, sensitive, flexible, and easy to use. These developments have made QELS/DLS an important tool in ophthalmic research where disease can be detected early and noninvasively before the clinical symptoms appear.

  14. Dynamics of poly(ethylene oxide) in a blend with poly(methyl methacrylate): A quasielastic neutron scattering and molecular dynamics simulations study

    International Nuclear Information System (INIS)

    Genix, A.-C.; Arbe, A.; Alvarez, F.; Colmenero, J.; Willner, L.; Richter, D.

    2005-01-01

    In this paper, we have addressed the question of the dynamic miscibility in a blend characterized by very different glass-transition temperatures, T g , for the components: poly(ethylene oxide) and poly(methyl methacrylate) (PEO/PMMA). The combination of quasielastic neutron scattering with isotopic labeling and fully atomistic molecular dynamics simulations has allowed us to selectively investigate the dynamics of the two components in the picosecond--10 nanoseconds scale at temperatures close and above the T g of the blend. The main focus was on the PEO component, i.e., that of the lowest T g , but first we have characterized the dynamics of the other component in the blend and of the pure PEO homopolymer as reference. In the region investigated, the dynamics of PMMA in the blend is strongly affected by the α-methyl rotation; an additional process detected in the experimental window 65 K above the blend-T g can be identified as the merged αβ process of this component that shows strong deviations from Gaussian behavior. On the other hand, pure PEO displays entropy driven dynamics up to very large momentum transfers. Such kind of motion seems to freeze when the PEO chains are in the blend. There, we have directly observed a very heterogeneous and moreover confined dynamics for the PEO component. The presence of the hardly moving PMMA matrix leads to the creation of little pockets of mobility where PEO can move. The characteristic size of such confined islands of mobility might be estimated to be of ≅1 nm. These findings are corroborated by the simulation study, which has been an essential support and guide in our data analysis procedure

  15. Quasi-elastic measurements using neutron spin flippers

    International Nuclear Information System (INIS)

    Bleuel, M.; Fitzsimmons, M.R.; Lal, J.

    2008-01-01

    A method for low-resolution quasi-elastic measurements using commonly available components on a polarized neutron beam reflectometer is demonstrated. By amplitude modulation of the current in a neutron spin flipper placed between the neutron beam polarizer and polarization analyzer, the intensity of the neutron beam illuminating a sample is similarly modulated (or chopped). We show that the intensity contrast between subsequent chopped pulses is dramatically reduced by a sample that changes neutron velocity

  16. Quasi-elastic Neutrino Scattering - an Overview

    International Nuclear Information System (INIS)

    Sobczyk, Jan T.

    2011-01-01

    A non-technical overview of charge current quasi-elastic neutrino interaction is presented. Many body computations of multinucleon ejection which is proposed to explain recent large axial mass measurements are discussed. A few comments on recent experimental results reported at NuInt11 workshop are included.

  17. A Measurement of the Neutron Electric Form Factor in Dvec ($\\vec{e}$,e'n)p Quasielastic Scattering at Q2=0.5(GeV/c)2

    Energy Technology Data Exchange (ETDEWEB)

    Zhu, Hongguo [Univ. of Virginia, Charlottesville, VA (United States)

    2000-08-01

    The form factors of the neutron give information on fundamental properties of the nucleons and provide a critical testing ground for models based on QCD. In late 1998, Jefferson Lab (JLAB) experiment E93-026 measured the spin-dependent part of the exclusive (e, e'n) scattering cross section from a polarized deuterated ammonia (15ND3) target at a four momentum transfer squared of Q2 = 0.5 (GeV/c)2. A longitudinally polarized electron beam was scattered from the polarized target and the quasi-elastically scattered electron was detected in coincidence with the knocked-out neutron. The data have been analyzed in terms of the spin-correlation parameter, or the electron-deuteron vector asymmetry (A$V\\atop{ed}$), of (e, e'n) to determine the neutron electric form factor G$n\\atop{E}$. The result is consistent with data from existing experiments and shows a good agreement with the Galster parameterization of G$n\\atop{E}$ within experimental uncertainty.

  18. Heavily doped M1−xUxF2+2x fluorites studied by quasielastic neutron scattering(M=Ba) and specific heat measurements (M=Pb)

    DEFF Research Database (Denmark)

    Andersen, Niels Hessel; Clausen, Kurt Nørgaard; Kjems, Jørgen

    1983-01-01

    of doping is an increase of the thermally generated defect concentration; at high temperatures the effect is reversed. The microscopic defect structure of Ba0.9U0.1F2.2 has been studied by diffuse quasielastic neutron scattering experiments at room temperature. The experimental observations are in good......The thermal generation of defects in pure and doped Pb1−xUxF2+2x (x=0, 0.05and0.10) has been studied by specific heat measurements between 475 k and 875 k. A simple phenomenological mean field thermodynamic model has been developed and used to interpret the data. At low temperatures the result...

  19. Studies of the dynamic properties of materials using neutron scattering

    International Nuclear Information System (INIS)

    Lovesey, S.W.; Windsor, C.G.

    1985-09-01

    The dynamic properties of materials using the neutron scattering technique is reviewed. The basic properties of both nuclear scattering and magnetic scattering are summarized. The experimental methods used in neutron scattering are described, along with access to neutron sources, and neutron inelastic instruments. Applied materials science using inelastic neutron scattering; rotational tunnelling of a methyl group; molecular diffusion from quasi-elastic scattering; and the diffusion of colloidal particles and poly-nuclear complexes; are also briefly discussed. (U.K.)

  20. Effective Spectral Function for Quasielastic Scattering on Nuclei

    OpenAIRE

    Bodek, A.; Christy, M. E.; Coopersmith, B.

    2014-01-01

    Spectral functions that are used in neutrino event generators to model quasielastic (QE) scattering from nuclear targets include Fermi gas, Local Thomas Fermi gas (LTF), Bodek-Ritchie Fermi gas with high momentum tail, and the Benhar-Fantoni two dimensional spectral function. We find that the $\

  1. Inclusive quasielastic and deep inelastic electron scattering at high energies

    International Nuclear Information System (INIS)

    Day, D.B.

    1990-01-01

    With high electron energies a kinematic regime can be reached where it will be possible to separate quasielastic and deep inelastic scattering. We present a short description of these processes which dominate the inclusive spectrum. Using the highest momentum transfer data available to guide our estimates, we give the kinematic requirements and the cross sections expected. These results indicate that inclusive scattering at high q has a yet unfilled potential. 18 refs., 13 figs

  2. Quasielastic scattering using the (p,n) reaction at 795 MeV

    International Nuclear Information System (INIS)

    Prout, D.L.

    1992-08-01

    A survey in nuclear mass and in momentum transfer of cross sections and analyzing powers in the quasielastic region has been made using the (p,n) reaction. The measurements were performed at an energy of 795 MeV at the Neutron Time of Flight Facility and the Weapons Neutron Research line at LAMPF. The (p,n) reaction isolates the isovector (rvec τ 1 · rvec τ 2 ) part of the nucleon nucleus interaction. Standard models of quasielastic scattering were able to describe the magnitude and shape of the double differential cross sections very well if account was taken of a significant background from double scattering. In contrast, the quasielastic response was shifted to much higher excitation energy than what was expected. This was true for all nuclei at moderate to large momenta transfers. Neither the Coulomb energy shift nor RPA calculations with the standard particle hole (p-h) interactions could account for this large shift. The data argue for a repulsive interaction in both the transverse and longitudinal channels of the p-h interaction. A suppression of the quasielastic analyzing power compared to the free nucleon nucleon analyzing power was found in nat C at all the angles measured. The same region in nat Pb showed little or no suppression. Part of the suppression in the nat C data may be accounted for by relativistic models of the nucleus employing large vector and scalar potentials with an effective mass of .85 times the free nucleon mass. The relatively larger contribution of double scattering nat Pb(rvec p, n) than to nat C(rvec p, n) may account for the difference in analyzing power for these two targets in the quasielastic region

  3. Quasi-elastic neutron line broadening in nematic liquid crystals

    International Nuclear Information System (INIS)

    Cvikl, B.; Dimic, V.; Dusic, M.; Kristof, E.; Srebotnjak, E.

    1979-01-01

    On the basis of a new random walk torsional oscillations model of the amplitude φ 0 of rigid flat molecules a quasi-elastic neutron line broadening has been calculated and the results compared to the measurements obtained on the sample of cholesteryl propionate. A good agreement was obtained. (author)

  4. Effective spectral function for quasielastic scattering on nuclei

    Energy Technology Data Exchange (ETDEWEB)

    Bodek, A.; Coopersmith, B. [University of Rochester, Department of Physics and Astronomy, Rochester, NY (United States); Christy, M.E. [Hampton University, Hampton, VA (United States)

    2014-10-15

    Spectral functions that are used in neutrino event, generators to model quasielastic (QE) scattering from nuclear targets include Fermi gas, Local Thomas Fermi gas (LTF), Bodek-Ritchie Fermi gas with high momentum tail, and the Benhar-Fantoni two dimensional spectral function. We find that the ν dependence of predictions of these spectral functions for the QE differential cross sections (d{sup 2}σ/dQ{sup 2}dν) are in disagreement with the prediction of the ψ' superscaling function which is extracted from fits to quasielastic electron scattering data on nuclear targets. It is known that spectral functions do not fully describe quasielastic scattering because they only model the initial state. Final state interactions distort the shape of the differential cross section at the peak and increase the cross section at the tails of the distribution. We show that the kinematic distributions predicted by the ψ' superscaling formalism can be well described with a modified effective spectral function (ESF). By construction, models using ESF in combination with the transverse enhancement contribution correctly predict electron QE scattering data. (orig.)

  5. Effective spectral function for quasielastic scattering on nuclei

    International Nuclear Information System (INIS)

    Bodek, A.; Coopersmith, B.; Christy, M.E.

    2014-01-01

    Spectral functions that are used in neutrino event, generators to model quasielastic (QE) scattering from nuclear targets include Fermi gas, Local Thomas Fermi gas (LTF), Bodek-Ritchie Fermi gas with high momentum tail, and the Benhar-Fantoni two dimensional spectral function. We find that the ν dependence of predictions of these spectral functions for the QE differential cross sections (d 2 σ/dQ 2 dν) are in disagreement with the prediction of the ψ' superscaling function which is extracted from fits to quasielastic electron scattering data on nuclear targets. It is known that spectral functions do not fully describe quasielastic scattering because they only model the initial state. Final state interactions distort the shape of the differential cross section at the peak and increase the cross section at the tails of the distribution. We show that the kinematic distributions predicted by the ψ' superscaling formalism can be well described with a modified effective spectral function (ESF). By construction, models using ESF in combination with the transverse enhancement contribution correctly predict electron QE scattering data. (orig.)

  6. Nucleon in nuclei from quasi-elastic electron scattering

    International Nuclear Information System (INIS)

    Gerard, A.

    1987-04-01

    One challenging problem in modern nuclear physics is to understand how the internal structure of the nucleon interferes with the dynamics of nucleons in a nucleus. The purpose of this paper is to review the present status of data in quasi-elastic electron scattering, to connect them with recent theoretical developments and to outline some future directions of research not accessible to present electron facilities

  7. Study of Quasielastic scattering for 7Li+159Tb at around- barrier energies

    Directory of Open Access Journals (Sweden)

    Mukherjee A.

    2017-01-01

    Full Text Available Quasielastic scattering cross sections for the reaction 7Li+159Tb have been measured at large backangles, at energies around the Coulomb barrier. The quasielastic barrier distribution has been extracted from the measured quasielastic scattering excitation function, including and excluding α particle contribution. The peak of the quasielastic barrier distribution including α particle contribution shows a shift towards higher energy compared to the peak of the distribution without α particles. The quasielastic barrier distribution when compared to the calculated fusion barrier distribution, appears to show reasonable agreement for the system.

  8. Dynamics of water and ions in clays of type montmorillonite by microscopic simulation and quasi-elastic neutron scattering; Dynamique de l'eau et des ions dans des argiles de type montmorillonite par simulation microscopique et diffusion quasi-elastique des neutrons

    Energy Technology Data Exchange (ETDEWEB)

    Malikova, N

    2005-09-15

    Montmorillonite clays in low hydration states, with Na{sup +} and Cs{sup +} compensating counter ions, are investigated by a combination of microscopic simulation and quasi-elastic neutron scattering to obtain information on the local structure and dynamics of water and ions in the interlayer. At first predictions of simulation into the dynamics of water and ions at elevate temperatures are shown (0 deg C 80 deg C, pertinent for the radioactive waste disposal scenario) Marked difference is observed between the modes of diffusion of the Na{sup +} and C{sup +} counter ions. In water dynamics, a significant step towards bulk water behaviour is seen on transition from the mono- to bilayer states. Secondly, a detailed comparison between simulation and quasi-elastic neutron scattering (Neutron Spin Echo and Time-of-Flight) regarding ambient temperature water dynamics is presented. Overall, the approaches are found to be in good agreement with each other and limitations of each of the methods are clearly shown. (author)

  9. Neutron scattering

    International Nuclear Information System (INIS)

    1991-02-01

    The annual report on hand gives an overview of the research work carried out in the Laboratory for Neutron Scattering (LNS) of the ETH Zuerich in 1990. Using the method of neutron scattering, it is possible to examine in detail the static and dynamic properties of the condensed material. In accordance with the multidisciplined character of the method, the LNS has for years maintained a system of intensive co-operation with numerous institutes in the areas of biology, chemistry, solid-state physics, crystallography and materials research. In 1990 over 100 scientists from more than 40 research groups both at home and abroad took part in the experiments. It was again a pleasure to see the number of graduate students present, who were studying for a doctorate and who could be introduced into the neutron scattering during their stay at the LNS and thus were in the position to touch on central ways of looking at a problem in their dissertation using this modern experimental method of solid-state research. In addition to the numerous and interesting ways of formulating the questions to explain the structure, nowadays the scientific programme increasingly includes particularly topical studies in connection with high temperature-supraconductors and materials research

  10. Selectron production in quasi-elastic electron-proton scattering

    International Nuclear Information System (INIS)

    Bartels, J.; Hollik, W.

    1985-08-01

    We calculate the cross section for the production of selectrons in quasi-elastic electron proton scattering at HERA energies. In the region of very small momentum transfer the cross section turns out to be large: e.g. sigma=36 pb for a selectron mass of 60 GeV, tsub(min) 2 ), and photino mass small compared to the selectron mass. Together with the clean experimental signature, this large cross section makes the reaction e+P->e+γ tilde+P one of the most promising HERA-processes in connection with the search for supersymmetric particles. (orig.)

  11. Quasi-elastic Scattering Measurements in the 6,7Li+144Sm Systems

    International Nuclear Information System (INIS)

    Capurro, O. A.; Arazi, A.; Fernandez Niello, J. O.; Figueira, J. M.; Marti, G. V.; Martinez Heimann, D.; Negri, A. E.; Pacheco, A. J.; Monteiro, D. S.; Otomar, D. R.; Gomes, P. R. S.; Guimaraes, V.

    2009-01-01

    In the present work, results of measurements of quasi-elastic scattering cross sections using a silicon-telescope detector at backward angles are reported. They allowed us to deduce fusion barrier distributions from the first derivative of the corresponding excitation function (-d(dσ qes /dσ Rut )/dE). We report data for the systems 6,7 Li on 144 Sm which are characterized by loosely bound projectiles onto a closed neutron shell target. The experimental excitation functions and the associated barrier distributions are compared for both systems.

  12. Neutron scattering. Lectures

    International Nuclear Information System (INIS)

    Brueckel, Thomas; Heger, Gernot; Richter, Dieter; Roth, Georg; Zorn, Reiner

    2012-01-01

    The following topics are dealt with: Neutron scattering in contemporary research, neutron sources, symmetry of crystals, diffraction, nanostructures investigated by small-angle neutron scattering, the structure of macromolecules, spin dependent and magnetic scattering, structural analysis, neutron reflectometry, magnetic nanostructures, inelastic scattering, strongly correlated electrons, dynamics of macromolecules, applications of neutron scattering. (HSI)

  13. Nuclear Transparency in Large Momentum Transfer Quasielastic Scattering

    International Nuclear Information System (INIS)

    Mardor, I.; Aclander, J.; Alster, J.; Kosonovsky, E.; Mardor, Y.; Navon, I.; Piasetzky, E.; Durrant, S.; Barton, D.; Bunce, G.; Carroll, A.; Gushue, S.; Makdisi, Y.; Roser, T.; Tanaka, M.; Christensen, N.; Courant, H.; Marshak, M.; White, C.; Heppelmann, S.; Minor, E.D.; Wu, J.; Nicholson, H.; Sutton, C.S.; Russell, J.

    1998-01-01

    We measured simultaneously pp elastic and quasielastic (p,2p) scattering in hydrogen, deuterium, and carbon for momentum transfers of 4.8 to 6.2 (GeV/c) 2 at incoming momenta of 5.9 and 7.5 GeV/c and center-of-mass scattering angles in the range θ c.m. =83.7 degree - 90 degree . The nuclear transparency is defined as the ratio of the quasielastic cross section to the free pp cross section. At incoming momentum of 5.9 GeV/c , the transparency of carbon decreases by a factor of 2 from θ c.m. ≅85 degree to θ c.m. ≅89 degree . At the largest angle the transparency of carbon increases from 5.9 to 7.5 GeV/c by more than 50%. The transparency in deuterium does not depend on incoming momentum nor on θ c.m. . copyright 1998 The American Physical Society

  14. Analysis of Quasi-Elastic e-n and e-p Scattering from Deuterium

    Science.gov (United States)

    Balsamo, Alexander; Gilfoyle, Gerard; CLAS12 Collaboration

    2017-09-01

    One of Jefferson Lab's goals is to unravel the quark-gluon structure of nuclei. We will use the ratio, R, of electron-neutron to electron-proton scattering on deuterium to probe the magnetic form factor of the neutron. We have developed an end-to-end analysis from simulation to extraction of R in quasi-elastic kinematics for an approved experiment with the CLAS12 detector. We focus on neutrons detected in the CLAS12 calorimeters and protons measured with the CLAS12 forward detector. Events were generated with the Quasi-Elastic Event Generator (QUEEG) and passed through the Monte Carlo code gemc to simulate the CLAS12 response. These simulated events were reconstructed using the latest CLAS12 Common Tools. We first match the solid angle for e-n and e-p events. The electron information is used to predict the path of both a neutron and proton through CLAS12. If both particles interact in CLAS12 the e-n and e-p events have the same solid angle. We select QE events by searching for nuclei near the predicted position. An angular cut between the predicted 3-momentum of the nucleon and the measured value, θpq, separates QE and inelastic events. We will show the simulated R as a function of the four-momentum transfer Q2. Work supported by the University of Richmond and the US Department of Energy.

  15. Final state effects in inclusive quasielastic electron scattering from nuclei: Clues from quantum fluids

    International Nuclear Information System (INIS)

    Silver, R.N.; Clark, J.W.

    1988-01-01

    The impulse approximation (IA) predicts that momentum distributions, n/sub k/, in many-body systems should be measurable by inclusive quasielastic scattering at high energy and momentum (w,Q) transfer. The observations that the cross section appears to satisfy ''Y-scaling'' (i.e., is a function not of both w and Q of a single variable, Y) is usually taken as a signature of the IA. In nuclear physics, inelastic electron scattering at GeV energies should reveal the high momentum components of the nuclear wave function. In quantum fluids, neutron scattering at hundreds of MeV energies should measure the Bose condensate in superfluid /sup 4/He and the Fermi surface discontinuity and depletion of the Fermi sea in /sup 3/He. In molecular and condensed matter systems, X-ray Compton scattering at keV energies reveals electronic n/sub k/. Such experiments test many-body wave functions calculated by methods such as Green Function and Path Integral Monte Carlo, and Fermi Hypernetted Chain. However, an outstanding issue has been the corrections to the IA due to the scattering of the recoiling particle from neighboring particles, which are termed ''final state effects'' (FSE). The FSE should be especially important in nuclei and quantum fluids where the potentials have steeply repulsive cores. While there have been a variety of theories proposed for FSE, until now none has been adequately tested by experiment. Recently, the ''hard core perturbation theory'' (HCPT) for FSE in quantum fluids by Silver has been successfully compared to new neutron scattering measurements on /sup 4/He by P. E. Sokol and colleagues. In this paper, we shall discuss the lessons of this success for the extraction of n/sub k/ in nuclei by inclusive ''quasielastic electron-nucleus scattering'' (QENS). 19 refs., 12 figs

  16. Neutron scattering. Lectures

    International Nuclear Information System (INIS)

    Brueckel, Thomas; Heger, Gernot; Richter, Dieter; Roth, Georg; Zorn, Reiner

    2013-01-01

    The following topics are dealt with: Neutron sources, symmetry of crystals, nanostructures investigated by small-angle neutron scattering, structure of macromolecules, spin dependent and magnetic scattering, structural analysis, neutron reflectometry, magnetic nanostructures, inelastic neutron scattering, strongly correlated electrons, polymer dynamics, applications of neutron scattering. (HSI)

  17. Neutron scattering. Lectures

    Energy Technology Data Exchange (ETDEWEB)

    Brueckel, Thomas; Heger, Gernot; Richter, Dieter; Roth, Georg; Zorn, Reiner (eds.)

    2010-07-01

    The following topics are dealt with: Neutron sources, neutron properties and elastic scattering, correlation functions measured by scattering experiments, symmetry of crystals, applications of neutron scattering, polarized-neutron scattering and polarization analysis, structural analysis, magnetic and lattice excitation studied by inelastic neutron scattering, macromolecules and self-assembly, dynamics of macromolecules, correlated electrons in complex transition-metal oxides, surfaces, interfaces, and thin films investigated by neutron reflectometry, nanomagnetism. (HSI)

  18. Neutron scattering. Lectures

    International Nuclear Information System (INIS)

    Brueckel, Thomas; Heger, Gernot; Richter, Dieter; Roth, Georg; Zorn, Reiner

    2010-01-01

    The following topics are dealt with: Neutron sources, neutron properties and elastic scattering, correlation functions measured by scattering experiments, symmetry of crystals, applications of neutron scattering, polarized-neutron scattering and polarization analysis, structural analysis, magnetic and lattice excitation studied by inelastic neutron scattering, macromolecules and self-assembly, dynamics of macromolecules, correlated electrons in complex transition-metal oxides, surfaces, interfaces, and thin films investigated by neutron reflectometry, nanomagnetism. (HSI)

  19. Neutron scattering. Lectures

    Energy Technology Data Exchange (ETDEWEB)

    Brueckel, Thomas; Heger, Gernot; Richter, Dieter; Roth, Georg; Zorn, Reiner [eds.

    2010-07-01

    The following topics are dealt with: Neutron sources, symmetry of crystals, diffraction, nanostructures investigated by small-angle neutron scattering, the structure of macromolecules, spin dependent and magnetic scattering, structural analysis, neutron reflectometry, magnetic nanostructures, inelastic scattering, strongly correlated electrons, dynamics of macromolecules, applications of neutron scattering. (HSI)

  20. Neutron scattering. Lectures

    International Nuclear Information System (INIS)

    Brueckel, Thomas; Heger, Gernot; Richter, Dieter; Roth, Georg; Zorn, Reiner

    2010-01-01

    The following topics are dealt with: Neutron sources, symmetry of crystals, diffraction, nanostructures investigated by small-angle neutron scattering, the structure of macromolecules, spin dependent and magnetic scattering, structural analysis, neutron reflectometry, magnetic nanostructures, inelastic scattering, strongly correlated electrons, dynamics of macromolecules, applications of neutron scattering. (HSI)

  1. Applications of thermal neutron scattering in biology, biochemistry and biophysics

    International Nuclear Information System (INIS)

    Worcester, D.L.

    1977-01-01

    Biological applications of thermal neutron scattering have increased rapidly in recent years. The following categories of biological research with thermal neutron scattering are presently identified: crystallography of biological molecules; neutron small-angle scattering of biological molecules in solution (these studies have already included numerous measurements of proteins, lippoproteins, viruses, ribosomal subunits and chromatin subunit particles); neutron small-angle diffraction and scattering from biological membranes and membrane components; and neutron quasielastic and inelastic scattering studies of the dynamic properties of biological molecules and materials. (author)

  2. Neutron scattering and physisorption

    International Nuclear Information System (INIS)

    Marlow, I.; Thomas, R.K.; Trewern, T.D.

    1977-01-01

    Neutron scattering experiments on methane and ammonia adsorbed on a graphitized carbon black are described. Diffraction from adsorbed deuterated methane shows that, at a coverage of 0.7, it forms an epitaxial layer with a √3x√3 structure. Between 50 and 60 K it undergoes a phase transition from two-dimensional solid to liquid (bulk melting point=89.7 K). Similar results are obtained for deuterated methane on a sample of graphon intercalated with potassium. From the effect of adsorbed methane on the intensities of 001 peaks of both substrates the carbon atom of the methane is estimated to be 3.3+-0.2 A from the surface. Ammonia-d 3 on graphon behaves quite differently from methane. It follows a type III isotherm and at low temperatures desorbs from the surface to form bulk ammonia. This has anomalous melting properties which are shown to be related to adsorption isobars for the system. The detailed interpretation of the results emphasizes the close link between adsorption and heterogeneous nucleation. Quasielastic experiments on the ammonia-graphon system show that the adsorbed ammonia is undergoing translational diffusion on the surface which is much faster than in the bulk. This is attributed to the breaking up of the hydrogen bonded network normally present in t

  3. New results of nuclear transparency to wide angle quasielastic scattering

    International Nuclear Information System (INIS)

    Mardor, I.

    1998-01-01

    We measured simultaneously pp elastic and quasi-elastic (p, 2p) scattering in hydro- gen, deuterium and carbon at incoming momenta of 5.9 and 7.5 GeV/c and center- of-mass scattering angles in the range 83.7 degrees to 90 degrees. We extracted the cross section ratios of quasi-elastic 12 C(p, 2p) to elastic 1 H(p, 2p) (C/H) and quasi-elastic D(p, 2p) to elastic 1 H(p, 2p) (D/H). The experiment was performed at the Brookhaven National Laboratory AGS accelerator using the EVA detector (experiment E850). For a detailed description of the experiment and the analysis. We determined that at incoming momentum of 5.9 GeV/c, the C/H ratio increases by a factor of 2 from θ cm = 89 degrees to θ cm 85 degrees, while at 7.5 GeV/c it is consistent with being flat. Further, at θ cm = 89 degrees the C/H ratio increases from 5.9 GeV/c to 7.5 GeV/c by more than 50%, while for lower θ cm the incoming momentum dependence is consistent with being flat. The rise of the C/H ratio with incoming momentum is similar to that observed in the previous measurement of the C/H ratio at θ cm near 90 degrees. The dependence of the C/H ratio on θ cm , was observed in our experiment for the first time. The D/H ratio does not depend on incoming momentum and θ cm Its absolute value is consistent with unity. The D/H ratio was measured in our experiment for the first time. The ratios discussed above are directly related to the nuclear transparency of 12 C and D. Nuclear transparency is a measure of the initial and final state interactions that the incoming and outgoing protons undergo before and after the main (p, 2p) reaction. The standard approach to nuclear transparency does not depend on the incoming momentum nor on θ cm in contradiction to the variation of the C/H ratio that we have observed. The incoming momentum dependence of the C/H ratio that we measured is similar to those of the inverse scaled pp differential cross section (s 10 (dσ/dt)) -1 where s and t are the Mandelstam variables

  4. Report of study meeting on nuclear physics of quasi-elastic scattering

    International Nuclear Information System (INIS)

    1992-10-01

    This meeting was held for three days from June 8 to 10, 1992, as one of the study meetings of Research Center for Nuclear Physics, Osaka University. The lectures were given on spin observables in quasi-elastic scattering, calculation of spin observables in 12 C, 40 Ca(p,n) reaction in quasifree scattering region, present state of quasi-elastic scattering, first results of (p,n) quasifree scattering with the new facility of the RCNP, spin-isospin response function and effect of Δ-hole configuration in finite nuclei, effective polarization of nuclei and observed amount of spin, (p,2p) measurement in the RCNP, quasi-elastic scattering in 2 H, 3 He and 4 He of polarized protons, quasifree Δ formation, 3 He(gamma, pπ ± ) reaction in Δ region, search for isobar components in 3 He by quasifree knockout studies, nonquasi-elastic process in photonuclear reaction, QF and NQF processes in gamma d→π + π - pn, coincidence scattering experiment in quasi-elastic scattering region, exclusive electron scattering of 3 He with full inclusion of final state interaction, quasi-elastic electron scattering and internucleon correlation and 13 other themes. (K.I.)

  5. Neutron scattering treatise on materials science and technology

    CERN Document Server

    Kostorz, G

    1979-01-01

    Treatise on Materials Science and Technology, Volume 15: Neutron Scattering shows how neutron scattering methods can be used to obtain important information on materials. The book discusses the general principles of neutron scattering; the techniques used in neutron crystallography; and the applications of nuclear and magnetic scattering. The text also describes the measurement of phonons, their role in phase transformations, and their behavior in the presence of crystal defects; and quasi-elastic scattering, with its special merits in the study of microscopic dynamical phenomena in solids and

  6. Neutron scattering

    International Nuclear Information System (INIS)

    Furrer, A.

    1993-01-01

    This report contains the text of 16 lectures given at the Summer School and the report on a panel discussion entitled ''the relative merits and complementarities of x-rays, synchrotron radiation, steady- and pulsed neutron sources''. figs., tabs., refs

  7. Neutron Scattering

    International Nuclear Information System (INIS)

    Fayer, Michael J.; Gee, Glendon W.

    2005-01-01

    The neutron probe is a standard tool for measuring soil water content. This article provides an overview of the underlying theory, describes the methodology for its calibration and use, discusses example applications, and identifies the safety issues. Soil water makes land-based life possible by satisfying plant water requirements, serving as a medium for nutrient movement to plant roots and nutrient cycling, and controlling the fate and transport of contaminants in the soil environment. Therefore, a successful understanding of the dynamics of plant growth, nutrient cycling, and contaminant behavior in the soil requires knowledge of the soil water content as well as its spatial and temporal variability. After more than 50 years, neutron probes remain the most reliable tool available for field monitoring of soil water content. Neutron probes provide integrated measurements over relatively large volumes of soil and, with proper access, allow for repeated sampling of the subsurface at the same locations. The limitations of neutron probes include costly and time-consuming manual operation, lack of data automation, and costly regulatory requirements. As more non-radioactive systems for soil water monitoring are developed to provide automated profiling capabilities, neutron-probe usage will likely decrease. Until then, neutron probes will continue to be a standard for reliable measurements of field water contents in soils around the globe

  8. Experimental study of the fusion dynamics of 32,34S + 197Au with quasi-elastic scattering

    International Nuclear Information System (INIS)

    Schuck, T.J.; Dasgupta, M.; Timmers, H.

    2000-01-01

    Full text: The fusion dynamics of heavy systems, such as 64 Ni + 208 Pb, leading to the synthesis of super-heavy elements is presently not fully understood. Typical beam energies in such reactions are of the order or smaller than the Coulomb barrier height to minimize the excitation energy of the compound system and increase the survival probability of evaporation residues. It is known that at such energies the relative motion of projectile and target couples to internal degrees of freedom of the system, such as collective motion and particle transfer. This can give rise to a distribution of fusion barriers, which generally leads to an enhancement of the fusion cross-section below the Coulomb barrier. The important role of the individual degrees of freedom can be identified by extracting representations of the barrier distribution from fusion excitation functions. Complementary representations can be obtained from measurements of the quasi-elastic or elastic scattering excitation functions at backward angles. The sensitivity of the representations from scattering is limited to the lower energy part of the barrier distribution, which, however, may contain important signatures of positive Q-value neutron transfer channels. Neutron transfer may be a precursor of neutron flow and neck-formation, which are considered in macroscopic models of the fusion of heavy systems. In order to study the influence of neutron transfer in heavy fusion reactions, quasielastic scattering has been measured for 32 , 34 S + 197 Au at energies spanning the Coulomb barrier. The quasi-elastic yield, including inelastic and transfer reactions, was detected at 165 deg with a Si-surface barrier detector. The excitation functions have been normalized to Rutherford scattering, detected at 30 deg using an existing gas ionisation detector. Representations of the barrier distributions have been extracted and are compared with earlier measurements for 32 S + 208 Pb

  9. Neutron Scattering Software

    Science.gov (United States)

    Home Page | Facilities | Reference | Software | Conferences | Announcements | Mailing Lists Neutron Scattering Banner Neutron Scattering Software A new portal for neutron scattering has just been established sets KUPLOT: data plotting and fitting software ILL/TAS: Matlab probrams for analyzing triple axis data

  10. Polarized Neutron Scattering

    OpenAIRE

    Roessli, B.; Böni, P.

    2000-01-01

    The technique of polarized neutron scattering is reviewed with emphasis on applications. Many examples of the usefulness of the method in various fields of physics are given like the determination of spin density maps, measurement of complex magnetic structures with spherical neutron polarimetry, inelastic neutron scattering and separation of coherent and incoherent scattering with help of the generalized XYZ method.

  11. Analysing power for quasi-elastic pp scattering in carbon and for elastic pp scattering on free protons

    International Nuclear Information System (INIS)

    Bystricky, J.; Deregel, J.; Lehar, F.

    1984-01-01

    The ratio of the analysing powers for quasi-elastic pp scattering in carbon and for elastic scattering on free protons was measured from T = 0.52 to 2.8 GeV by scattering of the SATURNE II polarized proton beam on carbon and CH 2 . It was found to have a maximum at about 0.8 GeV. The energy dependence for quasi-elastic scattering on carbon had not been measured before above 1 GeV. The observed effect was not expected from simple models

  12. Modifications of nucleons in nuclei in quasi-elastic electron-nucleus scattering

    International Nuclear Information System (INIS)

    Mulders, P.J.

    1988-01-01

    In inelastic electron scattering two scaling regions are observed in which the scattering is dominated by quasi-elastic scattering. For large momentum transfers, √Q 2 > 2 GeV/c, the scattering process is dominated by quasi-elastic scattering off quarks, whereas for √Q 2 ≅ 0.5 GeV/c the dominant contribution is quasi-elastic scattering off nucleons. This corresponds nicely to our first order picture of the nucleus consisting of nucleons, which in turn are composed of quarks. In the nucleon-scaling region, possible modifications of nucleon properties show up through a study of the Q 2 dependence and the relative strength of the transverse and longitudinal cross sections. Results of both inclusive (e,e') and exclusive (e,e'p) experiments in the quasi-elastic scattering region indeed show a behavior that could indicate modifications of intrinsic properties of individual nucleons in the nucleus, although the question remains if one has correctly disentangled the effects of the (long range) interactions between nucleons and those connected to the internal structure of nucleons. Even so, a simple (one-parameter) size rescaling for nucleons appears to be inconsistent with the data and also with some known conventional nuclear physics observables. Therefore the inclusion of two-nucleon correlations appears necessary in order to be able to understand the data. Such correlations can for instance be due to the effect of the Pauli principle on the quark level. (orig.)

  13. Inelastic neutron scattering from non-framework species within zeolites

    International Nuclear Information System (INIS)

    Newsam, J.M.; Brun, T.O.; Trouw, F.; Iton, L.E.; Curtiss, L.A.

    1990-01-01

    Inelastic and quasielastic neutron scattering have special advantages for studying certain of the motional properties of protonated or organic species within zeolites and related microporous materials. In this paper these advantages and various experimental methods are outlined, and illustrated by measurements of torsional vibrations and rotational diffusion of tetramethylammonium (TMA) cations occluded within zeolites TMA-sodalite, omega, ZK-4 and SAPO-20

  14. Neutron scattering and magnetism

    International Nuclear Information System (INIS)

    Mackintosh, A.R.

    1983-01-01

    Those properties of the neutron which make it a unique tool for the study of magnetism are described. The scattering of neutrons by magnetic solids is briefly reviewed, with emphasis on the information on the magnetic structure and dynamics which is inherent in the scattering cross-section. The contribution of neutron scattering to our understanding of magnetic ordering, excitations and phase transitions is illustrated by experimental results on a variety of magnetic crystals. (author)

  15. Thermal-neutron multiple scattering: critical double scattering

    International Nuclear Information System (INIS)

    Holm, W.A.

    1976-01-01

    A quantum mechanical formulation for multiple scattering of thermal-neutrons from macroscopic targets is presented and applied to single and double scattering. Critical nuclear scattering from liquids and critical magnetic scattering from ferromagnets are treated in detail in the quasielastic approximation for target systems slightly above their critical points. Numerical estimates are made of the double scattering contribution to the critical magnetic cross section using relevant parameters from actual experiments performed on various ferromagnets. The effect is to alter the usual Lorentzian line shape dependence on neutron wave vector transfer. Comparison with corresponding deviations in line shape resulting from the use of Fisher's modified form of the Ornstein-Zernike spin correlations within the framework of single scattering theory leads to values for the critical exponent eta of the modified correlations which reproduce the effect of double scattering. In addition, it is shown that by restricting the range of applicability of the multiple scattering theory from the outset to critical scattering, Glauber's high energy approximation can be used to provide a much simpler and more powerful description of multiple scattering effects. When sufficiently close to the critical point, it provides a closed form expression for the differential cross section which includes all orders of scattering and has the same form as the single scattering cross section with a modified exponent for the wave vector transfer

  16. Position calibration of silicon strip detector using quasi-elastic scattering of 16O+197Au

    International Nuclear Information System (INIS)

    Yan Wenqi; Hu Hailong; Zhang Gaolong

    2013-01-01

    Background: Elastic scattering is induced by weakly unstable nuclei. Generally, a good angular resolution for angular distribution of elastic scattering is needed. The silicon strip detector is often used for this kind of experiment. Purpose: In order to use silicon strip detector to study the elastic scattering of weakly unbound nuclei, it is important to get the information of its position calibration. It is well known that the elastic scattering of stable nuclei has a good angular distribution and many experimental data have been obtained. Methods: So the scattering of stable nuclei can be used to calibrate the position information of silicon strip detector. In this experiment, the positions of silicon strip detectors are calibrated using 101 MeV and 59 MeV 16 O scattering on the 197 Au target. Results: The quasi-elastic peaks can be observed in the silicon strip detectors and the counts of quasi-elastic 16 O can be obtained. The solid angles of the silicon strip detectors are calibrated by using alpha source which has three alpha energy values. The angular distribution of quasi-elastic scattering of 16 O+ 197 Au is obtained at these two energy values. Conclusions: The experimental data of angular distribution are reasonable and fit for the principle of angular distribution of elastic scattering. It is concluded that in the experiment these silicon strip detectors can accurately give the position information and can be used for the elastic scattering experiment. (authors)

  17. Quantum Monte Carlo calculation of neutral-current ν -12C inclusive quasielastic scattering

    Science.gov (United States)

    Lovato, A.; Gandolfi, S.; Carlson, J.; Lusk, Ewing; Pieper, Steven C.; Schiavilla, R.

    2018-02-01

    Quasielastic neutrino scattering is an important aspect of the experimental program to study fundamental neutrino properties including neutrino masses, mixing angles, mass hierarchy, and charge-conjugation parity (CP)- violating phase. Proper interpretation of the experiments requires reliable theoretical calculations of neutrino-nucleus scattering. In this paper we present calculations of response functions and cross sections by neutral-current scattering of neutrinos off 12C. These calculations are based on realistic treatments of nuclear interactions and currents, the latter including the axial, vector, and vector-axial interference terms crucial for determining the difference between neutrino and antineutrino scattering and the CP-violating phase. We find that the strength and energy dependence of two-nucleon processes induced by correlation effects and interaction currents are crucial in providing the most accurate description of neutrino-nucleus scattering in the quasielastic regime.

  18. Nuclear re-interaction effects in quasi-elastic neutrino nucleus scattering

    Energy Technology Data Exchange (ETDEWEB)

    Co, G.; Bleve, C.; De Mitri, I.; Martello, D

    2002-11-01

    The quasi-elastic {nu}-nucleus cross section has been calculated by using a Fermi gas model corrected to consider the re-scattering between the emitted nucleon and the rest nucleus. As an example of the relevance of this effect we show results for the muon production cross section on {sup 16}O target.

  19. Solution structure of a short dna fragment studied by neutron scattering

    DEFF Research Database (Denmark)

    Lederer, H.; May, R. P.; Kjems, Jørgen

    1986-01-01

    -DNA. The neutron scattering curve is well fitted by that of a rigid rod with a length of 44 nm and a diameter of 2 nm. The result were confirmed by quasi-elastic light scattering and analytical centrifugation. The neutron measurements in H2O and D2O buffer reveal a cross-sectional in homogeneity not detected by X...

  20. Small angle neutron scattering (SANS) under non-equilibrium conditions

    International Nuclear Information System (INIS)

    Oberthur, R.C.

    1984-01-01

    The use of small angle neutron scattering (SANS) for the study of systems under non-equilibrium conditions is illustrated by three types of experiments in the field of polymer research: - the relaxation of a system from an initial non-equilibrium state towards equilibrium, - the cyclic or repetitive installation of a series of non-equilibrium states in a system, - the steady non-equilibrium state maintained by a constant dissipation of energy within the system. Characteristic times obtained in these experiments with SANS are compared with the times obtained from quasi-elastic neutron and light scattering, which yield information about the equilibrium dynamics of the system. The limits of SANS applied to non-equilibrium systems for the measurement of relaxation times at different length scales are shown and compared to the limits of quasielastic neutron and light scattering

  1. Diffuse scattering of neutrons

    International Nuclear Information System (INIS)

    Novion, C.H. de.

    1981-02-01

    The use of neutron scattering to study atomic disorder in metals and alloys is described. The diffuse elastic scattering of neutrons by a perfect crystal lattice leads to a diffraction spectrum with only Bragg spreads. the existence of disorder in the crystal results in intensity and position modifications to these spreads, and above all, to the appearance of a low intensity scatter between Bragg peaks. The elastic scattering of neutrons is treated in this text, i.e. by measuring the number of scattered neutrons having the same energy as the incident neutrons. Such measurements yield information on the static disorder in the crystal and time average fluctuations in composition and atomic displacements [fr

  2. Neutron scattering. Experiment manuals

    Energy Technology Data Exchange (ETDEWEB)

    Brueckel, Thomas; Heger, Gernot; Richter, Dieter; Roth, Georg; Zorn, Reiner (eds.)

    2010-07-01

    The following topics are dealt with: The thermal triple axis spectrometer PUMA, the high-resolution powder diffractometer SPODI, the hot single-crystal diffractometer HEiDi for structure analysis with neutrons, the backscattering spectrometer SPHERES, neutron polarization analysis with tht time-of-flight spectrometer DNS, the neutron spin-echo spectrometer J-NSE, small-angle neutron scattering with the KWS-1 and KWS-2 diffractometers, the very-small-angle neutron scattering diffractrometer with focusing mirror KWS-3, the resonance spin-echo spectrometer RESEDA, the reflectometer TREFF, the time-of-flight spectrometer TOFTOF. (HSI)

  3. Neutron scattering. Experiment manuals

    International Nuclear Information System (INIS)

    Brueckel, Thomas; Heger, Gernot; Richter, Dieter; Roth, Georg; Zorn, Reiner

    2010-01-01

    The following topics are dealt with: The thermal triple axis spectrometer PUMA, the high-resolution powder diffractometer SPODI, the hot single-crystal diffractometer HEiDi for structure analysis with neutrons, the backscattering spectrometer SPHERES, neutron polarization analysis with tht time-of-flight spectrometer DNS, the neutron spin-echo spectrometer J-NSE, small-angle neutron scattering with the KWS-1 and KWS-2 diffractometers, the very-small-angle neutron scattering diffractrometer with focusing mirror KWS-3, the resonance spin-echo spectrometer RESEDA, the reflectometer TREFF, the time-of-flight spectrometer TOFTOF. (HSI)

  4. Scattering with polarized neutrons

    International Nuclear Information System (INIS)

    Schweizer, J.

    2007-01-01

    In the history of neutron scattering, it was shown very soon that the use of polarized neutron beams brings much more information than usual scattering with unpolarized neutrons. We shall develop here the different scattering methods that imply polarized neutrons: 1) polarized beams without polarization analysis, the flipping ratio method; 2) polarized beams with a uniaxial polarization analysis; 3) polarized beams with a spherical polarization analysis. For all these scattering methods, we shall give examples of the physical problems which can been solved by these methods, particularly in the field of magnetism: investigation of complex magnetic structures, investigation of spin or magnetization densities in metals, insulators and molecular compounds, separation of magnetic and nuclear scattering, investigation of magnetic properties of liquids and amorphous materials and even, for non magnetic material, separation between coherent and incoherent scattering. (author)

  5. Quasielastic 3Hp scattering at 2.5 GeV/c triton momentum

    International Nuclear Information System (INIS)

    Blinov, A.V.; Chuvilo, I.V.; Ergakov, V.A.

    1982-01-01

    The differential cross sections of the quasielastic 3 Hp-scattering at a 2.5 GeV/c tritium momentum (Tsub(p)=318 MeV) have been measured using the ITEP 80 cm hydrogen buble chamber. The experimental results are compared with the predictions of the Glauber-Sitenke multiple scattering theory combined with the the completeness condition for the excited nucleus wave functions. The validity of the Glauber sum rule for the differential cross sections is investigated

  6. Introduction to neutron scattering

    Energy Technology Data Exchange (ETDEWEB)

    Fischer, W E [Paul Scherrer Inst. (PSI), Villigen (Switzerland)

    1996-11-01

    We give here an introduction to the theoretical principles of neutron scattering. The relationship between scattering- and correlation-functions is particularly emphasized. Within the framework of linear response theory (justified by the weakness of the basic interaction) the relation between fluctuation and dissipation is discussed. This general framework explains the particular power of neutron scattering as an experimental method. (author) 4 figs., 4 refs.

  7. Neutron-proton scattering

    International Nuclear Information System (INIS)

    Doll, P.

    1990-02-01

    Neutron-proton scattering as fundamental interaction process below and above hundred MeV is discussed. Quark model inspired interactions and phenomenological potential models are described. The seminar also indicates the experimental improvements for achieving new precise scattering data. Concluding remarks indicate the relevance of nucleon-nucleon scattering results to finite nuclei. (orig.) [de

  8. Polarimetric neutron scattering

    International Nuclear Information System (INIS)

    Tasset, F.

    2001-01-01

    Polarimetric Neutron Scattering in introduced, both by, explaining methodological issues and the corresponding instrumental developments. After a short overview of neutron spin polarization and the neutron polarization 3d-vector a pictorial approach of the microscopic theory is used to show how a polarized beam interacts with lattice and magnetic Fourier components in a crystal. Examples are given of using Spherical Neutron Polarimetry (SNP) and the corresponding Cryopad polarimeter for the investigation of non-collinear magnetic structures. (R.P.)

  9. CRPA calculations for neutrino-nucleus scattering. From very low energies to the quasielastic peak

    International Nuclear Information System (INIS)

    Jachowicz, Natalie; Pandey, Vishvas; Martini, Marco; Gonzalez-Jimenez, Raul; Van Cuyck, Tom; Van Dessel, Nils

    2016-01-01

    We present continuum random phase approximation calculations (CRPA) for neutrino-induced quasielastic scattering off atomic nuclei. The validity of our formalism is checked by a careful confrontation of its results with semi-inclusive double-differential electron scattering data. We pay special attention to excitations in the giant resonance region. The CRPA is well-suited for the description of interactions in this energy range. We aim at providing a uniform description of one-nucleon knockout processes over the whole energy range from threshold to the quasielastic peak. Our calculations point to the fact that low-energy and giant-resonance excitations provide a non-negligible contribution to the interaction strength, especially at forward lepton-scattering angles. (author)

  10. Virtual neutron scattering experiments

    DEFF Research Database (Denmark)

    Overgaard, Julie Hougaard; Bruun, Jesper; May, Michael

    2017-01-01

    . In the last week of the course, students travel to a large-scale neutron scattering facility to perform real neutron scattering experiments. Through student interviews and survey answers, we argue, that the virtual training prepares the students to engage more fruitfully with experiments by letting them focus......We describe how virtual experiments can be utilized in a learning design that prepares students for hands-on experiments at large-scale facilities. We illustrate the design by showing how virtual experiments are used at the Niels Bohr Institute in a master level course on neutron scattering...

  11. Deep inelastic neutron scattering

    International Nuclear Information System (INIS)

    Mayers, J.

    1989-03-01

    The report is based on an invited talk given at a conference on ''Neutron Scattering at ISIS: Recent Highlights in Condensed Matter Research'', which was held in Rome, 1988, and is intended as an introduction to the techniques of Deep Inelastic Neutron Scattering. The subject is discussed under the following topic headings:- the impulse approximation I.A., scaling behaviour, kinematical consequences of energy and momentum conservation, examples of measurements, derivation of the I.A., the I.A. in a harmonic system, and validity of the I.A. in neutron scattering. (U.K.)

  12. Neutron scattering. Experiment manuals

    International Nuclear Information System (INIS)

    Brueckel, Thomas; Heger, Gernot; Richter, Dieter; Roth, Georg; Zorn, Reiner

    2014-01-01

    The following topics are dealt with: The thermal triple-axis spectrometer PUMA, the high-resolution powder diffractometer SPODI, the hot-single-crystal diffractometer HEiDi, the three-axis spectrometer PANDA, the backscattering spectrometer SPHERES, the DNS neutron-polarization analysis, the neutron spin-echo spectrometer J-NSE, small-angle neutron scattering at KWS-1 and KWS-2, a very-small-angle neutron scattering diffractometer with focusing mirror, the reflectometer TREFF, the time-of-flight spectrometer TOFTOF. (HSI)

  13. Studies of molecular dynamics with neutron scattering techniques. Part of a coordinated programme on neutron scattering techniques

    International Nuclear Information System (INIS)

    Vinhas, L.A.

    1980-05-01

    Molecular dynamics was studied in samples of tert-butanol, cyclohexanol and methanol, using neutron inelastic and quasi-elastic techniques. The frequency spectra of cyclohexanol in crystalline phase were interpreted by assigning individual energy peaks to hindered rotation of molecules, lattice vibration, hydrogen bond stretching and ring bending modes. Neutron quasi-elastic scattering measurements permitted the testing of models for molecular diffusion as a function of temperature. The interpretation of neutron incoherent inelastic scattering on methanol indicated the different modes of molecular dynamics in this material; individual inelastic peaks in the spectra could be assigned to vibrations of crystalline lattice, stretching of hydrogen bond and vibrational and torsional modes of CH 3 OH molecule. The results of the experimental work on tertbutanol indicate two distinct modes of motion in this material: individual molecular librations are superposed to a cooperative rotation diffusion which occurs both in solid and in liquid state

  14. Symposium on neutron scattering

    International Nuclear Information System (INIS)

    Lehmann, M.S.; Saenger, W.; Hildebrandt, G.; Dachs, H.

    1984-01-01

    Extended abstracts of the named symposium are presented. The first part of this report contains the abstracts of the lectures, the second those of the posters. Topics discussed on the symposium include neutron diffraction and neutron scattering studies in magnetism, solid state chemistry and physics, materials research. Some papers discussing instruments and methods are included too. (GSCH)

  15. Introductory theory of neutron scattering

    International Nuclear Information System (INIS)

    Gunn, J.M.F.

    1986-12-01

    The paper comprises a set of six lecture notes which were delivered to the summer school on 'Neutron Scattering at a pulsed source', Rutherford Laboratory, United Kingdom, 1986. The lectures concern the physical principles of neutron scattering. The topics of the lectures include: diffraction, incoherent inelastic scattering, connection with the Schroedinger equation, magnetic scattering, coherent inelastic scattering, and surfaces and neutron optics. (UK)

  16. Incoherent neutron scattering functions for random jump diffusion in bounded and infinite media

    International Nuclear Information System (INIS)

    Hall, P.L.; Ross, D.K.

    1981-01-01

    The incoherent neutron scattering function for unbounded jump diffusion is calculated from random walk theory assuming a gaussian distribution of jump lengths. The method is then applied to calculate the scattering function for spatially bounded random jumps in one dimension. The dependence on momentum transfer of the quasi-elastic energy broadenings predicted by this model and a previous model for bounded one-dimensional continuous diffusion are calculated and compared with the predictions of models for diffusion in unbounded media. The one-dimensional solutions can readily be generalized to three dimensions to provide a description of quasi-elastic scattering of neutrons by molecules undergoing localized random motions. (author)

  17. Cluster folding-model for quasi-elastic scattering of 23Na from 208Pb

    International Nuclear Information System (INIS)

    Kabir, A.; Johnson, R.C.; Tostevin, M.H.

    1991-01-01

    A cluster model of 23 Na is used to calculate the 23 Na-target interaction potentials by folding the cluster wavefunction with the cluster-target interaction potentials. Coupled channels calculations are carried out for the quasi-elastic scattering of polarized 23 Na from 208 Pb at 170 MeV and compared with recent experiments. Qualitative agreement with experiment is obtained when the interaction is adjusted by a single overall normalization constant. (author)

  18. Studies of Water by Scattering of Slow Neutrons

    International Nuclear Information System (INIS)

    Skoeld, K.; Pilcher, E.; Larsson, K.E.

    1964-01-01

    The quasielastic scattering peak in light water at room temperature has been studied with neutrons of energy ∼ 5x10 -3 eV. The width and shape of the peak has been determined by the time-of-flight technique at two scattering angles. If it is assumed that the broad inelastic spectrum is due to scattering by a monoatomic gas of mass 18, it is found that the quasielastic scattering is in good agreement with the predictions by the continuous diffusion model. Inelastic spectra were recorded up to 13x10 -3 eV. Indications of two discrete energy transfers (8 and 14x10 -4 eV) are observed in the 90 deg run. The results are discussed and compared with earlier observations

  19. Studies of Water by Scattering of Slow Neutrons

    Energy Technology Data Exchange (ETDEWEB)

    Skoeld, K; Pilcher, E; Larsson, K E

    1964-01-15

    The quasielastic scattering peak in light water at room temperature has been studied with neutrons of energy {approx} 5x10{sup -3} eV. The width and shape of the peak has been determined by the time-of-flight technique at two scattering angles. If it is assumed that the broad inelastic spectrum is due to scattering by a monoatomic gas of mass 18, it is found that the quasielastic scattering is in good agreement with the predictions by the continuous diffusion model. Inelastic spectra were recorded up to 13x10{sup -3} eV. Indications of two discrete energy transfers (8 and 14x10{sup -4} eV) are observed in the 90 deg run. The results are discussed and compared with earlier observations.

  20. MAGNETIC NEUTRON SCATTERING

    Energy Technology Data Exchange (ETDEWEB)

    ZALIZNYAK,I.A.; LEE,S.H.

    2004-07-30

    Much of our understanding of the atomic-scale magnetic structure and the dynamical properties of solids and liquids was gained from neutron-scattering studies. Elastic and inelastic neutron spectroscopy provided physicists with an unprecedented, detailed access to spin structures, magnetic-excitation spectra, soft-modes and critical dynamics at magnetic-phase transitions, which is unrivaled by other experimental techniques. Because the neutron has no electric charge, it is an ideal weakly interacting and highly penetrating probe of matter's inner structure and dynamics. Unlike techniques using photon electric fields or charged particles (e.g., electrons, muons) that significantly modify the local electronic environment, neutron spectroscopy allows determination of a material's intrinsic, unperturbed physical properties. The method is not sensitive to extraneous charges, electric fields, and the imperfection of surface layers. Because the neutron is a highly penetrating and non-destructive probe, neutron spectroscopy can probe the microscopic properties of bulk materials (not just their surface layers) and study samples embedded in complex environments, such as cryostats, magnets, and pressure cells, which are essential for understanding the physical origins of magnetic phenomena. Neutron scattering is arguably the most powerful and versatile experimental tool for studying the microscopic properties of the magnetic materials. The magnitude of the cross-section of the neutron magnetic scattering is similar to the cross-section of nuclear scattering by short-range nuclear forces, and is large enough to provide measurable scattering by the ordered magnetic structures and electron spin fluctuations. In the half-a-century or so that has passed since neutron beams with sufficient intensity for scattering applications became available with the advent of the nuclear reactors, they have became indispensable tools for studying a variety of important areas of modern

  1. Quasi-elastic shadowing in nucleus-nucleus elastic scattering

    Energy Technology Data Exchange (ETDEWEB)

    Dymarz, R; Malecki, A [Institute of Nuclear Physics, Krakow (Poland); Gluski, K [Institute of Nuclear Research, Warsaw (Poland); Picchi, P [Turin Univ. (Italy). Ist. di Fisica; Consiglio Nazionale delle Ricerche, Turin (Italy). Lab. di Cosmo-Geofisica)

    1979-01-06

    The complete evaluation of the Glauber multiple-scattering series for nucleus-nucleus collisions is a very difficult task and that is why various approximate formulae were proposed. In this work some of these approximations are discussed.

  2. Quasi-elastic helium-atom scattering from surfaces: experiment and interpretation

    International Nuclear Information System (INIS)

    Jardine, A.P.; Ellis, J.; Allison, W.

    2002-01-01

    Diffusion of an adsorbate is affected both by the adiabatic potential energy surface in which the adsorbate moves and by the rate of thermal coupling between the adsorbate and substrate. In principle both factors are amenable to investigation through quasi-elastic broadening in the energy spread of a probing beam of helium atoms. This review provides a topical summary of both the quasi-elastic helium-atom scattering technique and the available data in relation to the determination of diffusion parameters. In particular, we discuss the activation barriers deduced from experiment and their relation to the adiabatic potential and the central role played by the friction parameter, using the CO/Cu(001) system as a case study. The main issues to emerge are the need for detailed molecular dynamics simulations in the interpretation of data and the desirability of significantly greater energy resolution in the experiments themselves. (author)

  3. Virtual neutron scattering experiments

    DEFF Research Database (Denmark)

    Overgaard, Julie Hougaard; Bruun, Jesper; May, Michael

    2016-01-01

    We describe how virtual experiments can be utilized in a learning design that prepares students for hands-on experiments at large-scale facilities. We illustrate the design by showing how virtual experiments are used at the Niels Bohr Institute in a master level course on neutron scattering....... In the last week of the course, students travel to a large-scale neutron scattering facility to perform real neutron scattering experiments. Through student interviews and survey answers, we argue, that the virtual training prepares the students to engage more fruitfully with experiments by letting them focus...... on physics and data rather than the overwhelming instrumentation. We argue that this is because they can transfer their virtual experimental experience to the real-life situation. However, we also find that learning is still situated in the sense that only knowledge of particular experiments is transferred...

  4. Slow neutron scattering experiments

    International Nuclear Information System (INIS)

    Moon, R.M.

    1985-01-01

    Neutron scattering is a versatile technique that has been successfully applied to condensed-matter physics, biology, polymer science, chemistry, and materials science. The United States lost its leadership role in this field to Western Europe about 10 years ago. Recently, a modest investment in the United States in new facilities and a positive attitude on the part of the national laboratories toward outside users have resulted in a dramatic increase in the number of US scientists involved in neutron scattering research. Plans are being made for investments in new and improved facilities that could return the leadership role to the United States. 23 references, 4 figures, 3 tables

  5. Neutron scattering on partially deuterated polybutadiene

    CERN Document Server

    Kahle, S; Monkenbusch, M; Richter, D; Arbe, A; Colmenero, J; Frick, B

    2002-01-01

    The molecular nature of the secondary relaxation (Johari-Goldstein relaxation) and its relationship with the alpha relaxation is in most cases still unknown. In order to access these processes on a molecular level, it is necessary to obtain spatial information of the relaxation. Through the momentum-transfer dependence of the dynamic structure factor S(Q,t), this information can be provided by quasielastic neutron scattering techniques. The large difference in scattering lengths between hydrogen and deuterium allows us to accentuate specific correlations between atoms in a polymer melt. Here, we report on recent results on a polybutadiene melt, where the double bond was hydrogeneous, while the methylene groups carried deuterons (d4h2-PB). In this way the correlations between the double bonds are emphasised. We will show that the double bond/double bond correlation function, generated in this way, shows the same temperature dependence as the viscosity at higher temperatures at the structure factor peak maximum...

  6. Neutron scattering in Australia

    International Nuclear Information System (INIS)

    Knott, R.B.

    1994-01-01

    Neutron scattering techniques have been part of the Australian scientific research community for the past three decades. The High Flux Australian Reactor (HIFAR) is a multi-use facility of modest performance that provides the only neutron source in the country suitable for neutron scattering. The limitations of HIFAR have been recognized and recently a Government initiated inquiry sought to evaluate the future needs of a neutron source. In essence, the inquiry suggested that a delay of several years would enable a number of key issues to be resolved, and therefore a more appropriate decision made. In the meantime, use of the present source is being optimized, and where necessary research is being undertaken at major overseas neutron facilities either on a formal or informal basis. Australia has, at present, a formal agreement with the Rutherford Appleton Laboratory (UK) for access to the spallation source ISIS. Various aspects of neutron scattering have been implemented on HIFAR, including investigations of the structure of biological relevant molecules. One aspect of these investigations will be presented. Preliminary results from a study of the interaction of the immunosuppressant drug, cyclosporin-A, with reconstituted membranes suggest that the hydrophobic drug interdigitated with lipid chains

  7. Neutron scattering in Australia

    Energy Technology Data Exchange (ETDEWEB)

    Knott, R.B. [Australian Nuclear Science and Technology Organisation, Menai (Australia)

    1994-12-31

    Neutron scattering techniques have been part of the Australian scientific research community for the past three decades. The High Flux Australian Reactor (HIFAR) is a multi-use facility of modest performance that provides the only neutron source in the country suitable for neutron scattering. The limitations of HIFAR have been recognized and recently a Government initiated inquiry sought to evaluate the future needs of a neutron source. In essence, the inquiry suggested that a delay of several years would enable a number of key issues to be resolved, and therefore a more appropriate decision made. In the meantime, use of the present source is being optimized, and where necessary research is being undertaken at major overseas neutron facilities either on a formal or informal basis. Australia has, at present, a formal agreement with the Rutherford Appleton Laboratory (UK) for access to the spallation source ISIS. Various aspects of neutron scattering have been implemented on HIFAR, including investigations of the structure of biological relevant molecules. One aspect of these investigations will be presented. Preliminary results from a study of the interaction of the immunosuppressant drug, cyclosporin-A, with reconstituted membranes suggest that the hydrophobic drug interdigitated with lipid chains.

  8. Studies on biological macromolecules by neutron inelastic scattering

    International Nuclear Information System (INIS)

    Fujiwara, Satoru; Nakagawa, Hiroshi

    2013-01-01

    Neutron inelastic scattering techniques, including quasielastic and elastic incoherent neutron scattering, provide unique tools to directly measure the protein dynamics at a picosecond time scale. Since the protein dynamics at this time scale is indispensable to the protein functions, elucidation of the protein dynamics is indispensable for ultimate understanding of the protein functions. There are two complementary directions of the protein dynamics studies: one is to explore the physical basis of the protein dynamics using 'model' proteins, and the other is more biology-oriented. Examples of the studies on the protein dynamics with neutron inelastic scattering are described. The examples of the studies in the former direction include the studies on the dynamical transitions of the proteins, the relationship between the protein dynamics and the hydration water dynamics, and combined analysis of the protein dynamics with molecular dynamics simulation. The examples of the studies in the latter direction include the elastic incoherent and quasielastic neutrons scattering studies of actin. Future prospects of the studies on the protein dynamics with neutron scattering are briefly described. (author)

  9. Small angle neutron scattering

    International Nuclear Information System (INIS)

    Bernardini, G.; Cherubini, G.; Fioravanti, A.; Olivi, A.

    1976-09-01

    A method for the analysis of the data derived from neutron small angle scattering measurements has been accomplished in the case of homogeneous particles, starting from the basic theory without making any assumption on the form of particle size distribution function. The experimental scattering curves are interpreted with the aid the computer by means of a proper routine. The parameters obtained are compared with the corresponding ones derived from observations at the transmission electron microscope

  10. Quasielastic electron scattering: effect of relativistic nuclear potentials

    International Nuclear Information System (INIS)

    Do Dang, G.; Nguyen Van Giai.

    1983-11-01

    It is shown that a solution to the difficulty encountered in reproducing simultaneously the experimental longitudinal and transverse response functions deduced from deep inelastic electron scattering may be found in a consistent treatment of the electromagnetic interaction in a Dirac equation in which Lorentz scalar and vector potentials are explicitly introduced. Results for 12 C and 40 Ca are given and compared with experiments

  11. Cross section measurements for quasi-elastic neutrino-nucleus scattering with the MINOS near detector

    Energy Technology Data Exchange (ETDEWEB)

    Dorman, Mark Edward [Univ. College London, Bloomsbury (United Kingdom)

    2008-04-01

    The Main Injector Neutrino Oscillation Search (MINOS) is a long baseline neutrino oscillation experiment based at the Fermi National Accelerator Laboratory (FNAL) in Chicago, Illinois. MINOS measures neutrino interactions in two large iron-scintillator tracking/sampling calorimeters; the Near Detector on-site at FNAL and the Far Detector located in the Soudan mine in northern Minnesota. The Near Detector has recorded a large number of neutrino interactions and this high statistics dataset can be used to make precision measurements of neutrino interaction cross sections. The cross section for charged-current quasi-elastic scattering has been measured by a number of previous experiments and these measurements disagree by up to 30%. A method to select a quasi-elastic enriched sample of neutrino interactions in the MINOS Near Detector is presented and a procedure to fit the kinematic distributions of this sample and extract the quasi-elastic cross section is introduced. The accuracy and robustness of the fitting procedure is studied using mock data and finally results from fits to the MINOS Near Detector data are presented.

  12. Cross section measurements for quasi-elastic neutrino-nucleus scattering with the MINOS near detector

    International Nuclear Information System (INIS)

    Dorman, Mark Edward

    2008-01-01

    The Main Injector Neutrino Oscillation Search (MINOS) is a long baseline neutrino oscillation experiment based at the Fermi National Accelerator Laboratory (FNAL) in Chicago, Illinois. MINOS measures neutrino interactions in two large iron-scintillator tracking/sampling calorimeters; the Near Detector on-site at FNAL and the Far Detector located in the Soudan mine in northern Minnesota. The Near Detector has recorded a large number of neutrino interactions and this high statistics dataset can be used to make precision measurements of neutrino interaction cross sections. The cross section for charged-current quasi-elastic scattering has been measured by a number of previous experiments and these measurements disagree by up to 30%. A method to select a quasi-elastic enriched sample of neutrino interactions in the MINOS Near Detector is presented and a procedure to fit the kinematic distributions of this sample and extract the quasi-elastic cross section is introduced. The accuracy and robustness of the fitting procedure is studied using mock data and finally results from fits to the MINOS Near Detector data are presented

  13. Quasielastic nucleon scattering using polarized beams and targets

    International Nuclear Information System (INIS)

    Haeusser, O.

    1990-07-01

    Inelastic scattering of polarized intermediate energy nucleons to continuum nuclear states is discussed with emphasis on recent results. Spin momentum correlations of protons in polarized targets of 3 He were observed for the first time. Complete spin observables in (p,p') show effects of the nuclear spin-isospin response and of an NN interaction modified by the nuclear medium. A comparison of Gamow Teller and isovector M1 giant resonance strengths in the sd shell provides evidence for large meson exchange current effects in the M1. (Author) (37 refs., 2 tabs., 9 figs.)

  14. High-energy elastic and quasi-elastic deuteron-nucleus scattering

    International Nuclear Information System (INIS)

    Tekou, Amouzou

    1974-01-01

    A study is made of deuteron-nucleus elastic and quasi-elastic scattering and the connection between the opaque nucleus model and the Glauber model is pointed out. The contributions to different cross-sections of the collisions in which the nucleus, excited by one of the nucleons of the deuteron, is brought back to the ground state by the other nucleon is analysed. Coherent deuteron disintegration is found to be highly improbable when the target nucleus is heavy and incoherent disintegration accounts for nearly all the deuteron disintegration. Thus a correct comparison between theoretical and experimental data on proton stripping must take the incoherent deuteron disintegration into consideration

  15. Two particle–hole excitations in charged current quasielastic antineutrino-nucleus scattering

    International Nuclear Information System (INIS)

    Nieves, J.; Ruiz Simo, I.; Vicente Vacas, M.J.

    2013-01-01

    We evaluate the quasielastic and multinucleon contributions to the antineutrino-nucleus scattering cross section and compare our results with the recent MiniBooNE data. We use a local Fermi gas model that includes RPA correlations and gets the multinucleon part from a systematic many body expansion of the W boson selfenergy in the nuclear medium. The same model had been quite successful for the neutrino cross section and contains no new parameters. We have also analyzed the relevance of 2p2h events for the antineutrino energy reconstruction

  16. Short Range Correlations in Nuclei at Large xbj through Inclusive Quasi-Elastic Electron Scattering

    Energy Technology Data Exchange (ETDEWEB)

    Ye, Zhihong [Univ. of Virginia, Charlottesville, VA (United States)

    2013-12-01

    The experiment, E08-014, in Hall-A at Jefferson Lab aims to study the short-range correlations (SRC) which are necessary to explain the nuclear strength absent in the mean field theory. The cross sections for 2H, 3He, 4He, 12C, 40Ca and 48Ca, were measured via inclusive quasi-elastic electron scattering from these nuclei in a Q2 range between 0.8 and 2.8 (GeV/c)2 for x>1. The cross section ratios of heavy nuclei to 2H were extracted to study two-nucleon SRC for 1

  17. Quasi-elastic Charm Production In Neutrino-nucleon Scattering

    CERN Document Server

    Bischofberger, M

    2005-01-01

    A study of quasi elastic charm production in charged current neutrino-nucleon scattering is presented. A sample of about 1.3 million interactions recorded with the NOMAD detector in the CERN SPS wide band neutrino beam has been searched for quasi elastically produced charmed baryons ( L+c,Sc and S*c ). The search has been performed in two exclusive decay channels of the L+c, both including a L . Also, the semi-inclusive decay channels L+c,Sc,S *c→L+X have been studied. Kinematic selection criteria have been chosen in order to obtain samples enriched with quasi elastic charm events. Signal efficiencies and background expectations have been estimated by Monte Carlo simulations. The observed number of events in each searched channel has been found to agree with the background expectation from charged and neutral current reactions and an upper limit for the cross section has been derived. For the quasi elastic charm production cross section averaged over the neutrino energy spectrum (&lan...

  18. Implementing the correlated fermi gas nuclear model for quasielastic neutrino-nucleus scattering

    Science.gov (United States)

    Tockstein, Jameson

    2017-09-01

    When studying neutrino oscillations an understanding of charged current quasielastic (CCQE) neutrino-nucleus scattering is imperative. This interaction depends on a nuclear model as well as knowledge of form factors. Neutrino experiments, such as MiniBooNE, often use the Relativistic Fermi Gas (RFG) nuclear model. Recently, the Correlated Fermi Gas (CFG) nuclear model was suggested in, based on inclusive and exclusive scattering experiments at JLab. We implement the CFG model for CCQE scattering. In particular, we provide analytic expressions for this implementation that can be used to analyze current and future neutrino CCQE data. This project was supported through the Wayne State University REU program under NSF Grant PHY-1460853 and by the DOE Grant DE-SC0007983.

  19. Exchange current contributions to quasi-elastic electron scattering

    International Nuclear Information System (INIS)

    Conte, J.S. Jr.

    1981-01-01

    Because electromagnetic interactions are weak and well understood, inelastic electron scattering has been very useful in elucidating aspects of nuclear structure. In the region of large electron energy loss, an extremely simple reaction picture (quasi-free knockout of a single nucleon or electroproduction of an isobar) and a simple nuclear model (Fermi gas) have provided both a good fit to experimental data and a dynamical determination of the nuclear Fermi momentum (k/sub F/). However, there exists an anomalous region where this picture fails. Two body correlations have not seemed to help give any better agreement. We have investigated the following questions: Do exchange current processes contribute importantly in this region. Do they help produce agreement with experiment. Also, how do they effect our previous picture of quasifree knockout. We calculate the effects of exchange currents in this region using the standard Feynman graph rules. We have included all important long range exchange currents: pair, pionic, and isobar exchange currents. We found it necessary to make non-relativistic reductions of these currents in order to facilitate calculations. The resulting multidimensional integrals were done using Monte Carlo techniques. All exchange currents which were investigated were found to be appreciable in the anomalous region, and also important in the quasi-free peak region. Inclusion of these amplitudes would supply all of the missing cross section in the anomalous region: however, it would destroy the agreement between theory and experiment in the region of the quasi-free nucleon peak, and thereby cast suspicion on the aforementioned dynamical determination of k/sub F/

  20. Small angle neutron scattering

    Directory of Open Access Journals (Sweden)

    Cousin Fabrice

    2015-01-01

    Full Text Available Small Angle Neutron Scattering (SANS is a technique that enables to probe the 3-D structure of materials on a typical size range lying from ∼ 1 nm up to ∼ a few 100 nm, the obtained information being statistically averaged on a sample whose volume is ∼ 1 cm3. This very rich technique enables to make a full structural characterization of a given object of nanometric dimensions (radius of gyration, shape, volume or mass, fractal dimension, specific area… through the determination of the form factor as well as the determination of the way objects are organized within in a continuous media, and therefore to describe interactions between them, through the determination of the structure factor. The specific properties of neutrons (possibility of tuning the scattering intensity by using the isotopic substitution, sensitivity to magnetism, negligible absorption, low energy of the incident neutrons make it particularly interesting in the fields of soft matter, biophysics, magnetic materials and metallurgy. In particular, the contrast variation methods allow to extract some informations that cannot be obtained by any other experimental techniques. This course is divided in two parts. The first one is devoted to the description of the principle of SANS: basics (formalism, coherent scattering/incoherent scattering, notion of elementary scatterer, form factor analysis (I(q→0, Guinier regime, intermediate regime, Porod regime, polydisperse system, structure factor analysis (2nd Virial coefficient, integral equations, characterization of aggregates, and contrast variation methods (how to create contrast in an homogeneous system, matching in ternary systems, extrapolation to zero concentration, Zero Averaged Contrast. It is illustrated by some representative examples. The second one describes the experimental aspects of SANS to guide user in its future experiments: description of SANS spectrometer, resolution of the spectrometer, optimization of

  1. Intercomparison of lepton-nucleus scattering models in the quasielastic region

    Science.gov (United States)

    Sobczyk, Joanna E.

    2017-10-01

    I present a discussion of the models of nuclear effects used to describe the inclusive electron-nucleus scattering in the quasielastic (QE) peak region, aiming to compare them and to draw conclusions about their reliability when applied in neutrino-nucleus interactions. A basic motivation is to reduce the systematic errors in the neutrino oscillation experiments. I concentrate on the neutrino energy profile of the T2K experiment, which provides me with a region of the greatest importance in terms of the highest contribution to the charge-current quasielastic (CCQE) cross section. Only electron-nucleus data that overlap with this region is chosen. In order to clarify the analysis, I split the data sets into three groups and draw conclusions separately from each one of them. Six models are selected for this comparison: Benhar's spectral function with and without the final-state interactions (Benhar's SF + FSI); the Valencia spectral function (Valencia SF), for higher energy transfers only with the hole spectral function; the Giessen Boltzmann-Uehling-Uhlenbeck (GiBUU) model; and the local and global Fermi gas models. The latter two are included as a benchmark to quantify the roles of various nuclear effects. All six models are often used in neutrino scattering studies. A short theoretical description of each model is given. Although in the selected data sets the QE mechanism dominates, I also discuss the possible impact of the 2p2h and the Δ contributions.

  2. Quasi-elastic scattering of electrons from 40Ca at high momentum transfer

    International Nuclear Information System (INIS)

    Yates, T.C.

    1992-01-01

    Previous quasi-elastic electron scattering experiments have yielded seemingly inconsistent results when the integrated longitudinal strength is compared to calculations using the relativistic fermi gas model. Measurements made at Saclay on 12 C, 40 Ca, 48 Ca, 56 Fe, and 208 Pb indicated a smaller integrated longitudinal strength than expected on the basis of the relativistic fermi gas model. However, 238 U data taken at Bates showed nearly the full expected longitudinal strength at a momentum transfer of 550 MeV/c. This is one of the outstanding discrepancies in nuclear physics. Earlier experiments were hampered in that high momentum transfer could not be obtained at forward angles where the longtudinal strength is a large fraction of the total strength. The present experiment was designed to take advantage of the higher energy capability (greater than 800 MeV) at Bates recirculated linac in order to obtain momentum transfers greater than 600 MeV/c at a scattering angle of 45.5 degrees. Under these conditions the longitudinal strength is 40-75% of the total quasi-elastic strength

  3. Separating form factor and nuclear model effects in quasielastic neutrino-nucleus scattering

    Science.gov (United States)

    Wieske, Joseph

    2017-09-01

    When studying neutrino oscillations an understanding of charged current quasielastic (CCQE) neutrino-nucleus scattering is imperative. This interaction depends on a nuclear model as well as knowledge of form factors. In the past, CCQE data from the MiniBooNE experiment was analyzed assuming the Relativistic Fermi Gas (RFG) nuclear model, an axial dipole form factor in, and using the the z-expansion for the axial form factor in. We present the first analysis that combines a non-RFG nuclear model, in particular the Correlated Fermi Gas nuclear model (CFG) of, and the z expansion for the axial form factor. This will allow us to separate form factor and nuclear model effects in CCQE scattering. This project was supported through the Wayne State University REU program under NSF Grant PHY-1460853 and by the DOE Grant DE-SC0007983.

  4. Measurement of the parity violation in quasi-elastic electroweak electron-scattering from 9Be

    International Nuclear Information System (INIS)

    Achenbach, W.; Andresen, H.G.

    1987-01-01

    Measurement of the Parity Violation in Quasi-Elastic Electroweak Electron-Scattering from 9 Be in the energy range of about 300 MeV is fulfilled. The measurement of the parity violating asymmetry is obtained by a comparison of scattering for a + helicity beam to that for a - helicity beams. To permit a meaningful comparison required that the + helicity and the - helicity beams being identical in all other respects. Measurements at different energies and targets (hydrogen, deuterium) in the medium energy region will allow to determine α, β, γ, δ in a model-independent way. Regarding future experiments at the Mainz microtron cw accelerator, coincidence experiments will open new experimental possibilities for large solid angle detector systems

  5. A study of quasi-elastic muon (anti)neutrino scattering in he NOMAD experiment

    International Nuclear Information System (INIS)

    Lyubushkin, Vladimir

    2009-01-01

    We have studied the muon neutrino and antineutrino quasi-elastic (QEL) scattering reactions (v μ n→μ - p and v-bar μ p→μ + n using a set of experimental data collected by the NOMAD collaboration. We have performed measurements of the cross-section of these processes on a nuclear target (mainly Carbon) normalizing it to the total v μ (v-bar μ ) charged current cross-section. The results for the flux averaged QEL cross-sections in the (anti)neutrino energy interval 3-100 GeV are qel >v μ = (0.92±0.02(stat)±0.06(syst))x10 -38 cm 2 and qel >v-bar μ = (0.81±0.05(stat)±0.09(syst))x10 -38 cm 2 for neutrino and antineutrino, respectively. The axial mass parameter MA was extracted from the measured quasi-elastic neutrino cross-section. The corresponding result is M A = 1.05±0.02(stat)±0.06(syst) GeV. It is consistent with the axial mass values recalculated from the antineutrino cross-section and extracted from the pure Q 2 shape analysis of the high purity sample of v μ quasi-elastic 2-track events, but has smaller systematic error and should be quoted as the main result of this work. Our measured MA is found to be in good agreement with the world average value obtained in previous deuterium filled bubble chamber experiments. The NOMAD measurement of M A is lower than those recently published by K2K and MiniBooNE collaborations. However, within the large errors quoted by these experiments on M A , these results are compatible with the more precise NOMAD value.

  6. Neutron inelastic scattering experiments on the mixed-valent compound YbCuAl

    International Nuclear Information System (INIS)

    Mattens, W.C.M.; de Boer, F.R.; Murani, A.P.; Lander, G.H.

    1979-01-01

    The dynamical susceptibility of YbCuAl has been established by means of time of flight neutron scattering experiments. Non-Korringa behavior of the quasi-elastic line-width has been found and comparison with NMR data will be given

  7. Neutron scattering investigation of magnetic excitations at high energy transfers

    International Nuclear Information System (INIS)

    Loong, C.K.

    1984-01-01

    With the advance of pulsed spallation neutron sources, neutron scattering investigation of elementary excitations in magnetic materials can now be extended to energies up to several hundreds of MeV. We have measured, using chopper spectrometers and time-of-flight techniques, the magnetic response functions of a series of d and f transition metals and compounds over a wide range of energy and momentum transfer. In PrO 2 , UO 2 , BaPrO 3 and CeB 6 we observed crystal-field transitions between the magnetic ground state and the excited levels in the energy range from 40 to 260 MeV. In materials exhibiting spin-fluctuation or mixed-valent character such as Ce 74 Th 26 , on the other hand, no sharp crystal-field lines but a broadened quasielastic magnetic peak was observed. The line width of the quasielastic component is thought to be connected to the spin-fluctuation energy of the 4f electrons. The significance of the neutron scattering results in relation to the ground state level structure of the magnetic ions and the spin-dynamics of the f electrons is discussed. Recently, in a study of the spin-wave excitations in itinerant magnetic systems, we have extended the spin-wave measurements in ferromagnetic iron up to about 160 MeV. Neutron scattering data at high energy transfers are of particular interest because they provide direct comparison with recent theories of itinerant magnetism. 26 references, 7 figures

  8. Inelastic scattering of neutrons

    International Nuclear Information System (INIS)

    Sal'nikov, O.A.

    1984-06-01

    The paper reviews the main problems concerning the mechanism of the inelastic scatterings of neutrons by nuclei, concentrating on the different models which calculate the angular distributions. In the region of overlapping levels, both the compound nucleus mechanism and the preequilibrium Griffin (exciton) model are discussed, and their contribution relative to that of a direct mechanism is considered. The parametrization of the level density and of the nuclear moment of inertia are also discussed. The excitation functions of discrete levels are also presented, and the importance of elucidating their five structure (for practical calculations, such as for shielding) is pointed out

  9. Near- and subbarrier elastic and quasielastic scattering of the weakly bound 6Li projectile on 144Sm

    International Nuclear Information System (INIS)

    Monteiro, D. S.; Otomar, D. R.; Lubian, J.; Gomes, P. R. S.; Capurro, O. A.; Marti, G. V.; Arazi, A.; Figueira, J. M.; Heimann, D. Martinez; Negri, A. E.; Pacheco, A. J.; Niello, J. O. Fernandez; Guimaraes, V.

    2009-01-01

    High-precision data of backward-angle elastic and quasielastic scattering for the weakly bound 6 Li projectile on 144 Sm target at deep-sub-barrier, near-, and above-barrier energies were measured. From the deep-sub-barrier data, the surface diffuseness of the nuclear interacting potential was studied. Barrier distributions were extracted from the first derivatives of the elastic and quasielastic excitation functions. It is shown that sequential breakup through the first resonant state of the 6 Li is an important channel to be included in coupled-channels calculations, even at deep-sub-barrier energies

  10. Single Crystal Diffuse Neutron Scattering

    Directory of Open Access Journals (Sweden)

    Richard Welberry

    2018-01-01

    Full Text Available Diffuse neutron scattering has become a valuable tool for investigating local structure in materials ranging from organic molecular crystals containing only light atoms to piezo-ceramics that frequently contain heavy elements. Although neutron sources will never be able to compete with X-rays in terms of the available flux the special properties of neutrons, viz. the ability to explore inelastic scattering events, the fact that scattering lengths do not vary systematically with atomic number and their ability to scatter from magnetic moments, provides strong motivation for developing neutron diffuse scattering methods. In this paper, we compare three different instruments that have been used by us to collect neutron diffuse scattering data. Two of these are on a spallation source and one on a reactor source.

  11. Recent advances and open questions in neutrino-induced quasi-elastic scattering and single photon production

    Energy Technology Data Exchange (ETDEWEB)

    Garvey, G.T., E-mail: garvey@lanl.gov [Los Alamos National Laboratory, P.O. Box 1663, Los Alamos, NM 87545 (United States); Harris, D.A., E-mail: dharris@fnal.gov [Fermi National Accelerator Laboratory, P.O. Box 500, Batavia, IL, 60510-5011 (United States); Tanaka, H.A., E-mail: tanaka@phas.ubc.ca [Institute of Particle Physics and Department of Physics and Astronomy, University of British Columbia, 6224 Agricultural Road, Vancouver, BC V6T 1Z1 (Canada); Tayloe, R., E-mail: rtayloe@indiana.edu [Department of Physics, Indiana University, 727 E. Third St., Bloomington, IN 47405-7105 (United States); Zeller, G.P., E-mail: gzeller@fnal.gov [Fermi National Accelerator Laboratory, P.O. Box 500, Batavia, IL, 60510-5011 (United States)

    2015-06-15

    The study of neutrino–nucleus interactions has recently seen rapid development with a new generation of accelerator-based neutrino experiments employing medium and heavy nuclear targets for the study of neutrino oscillations. A few unexpected results in the study of quasi-elastic scattering and single photon production have spurred a revisiting of the underlying nuclear physics and connections to electron–nucleus scattering. A thorough understanding and resolution of these issues is essential for future progress in the study of neutrino oscillations. A recent workshop hosted by the Institute of Nuclear Theory at the University of Washington (INT-13-54W) examined experimental and theoretical developments in neutrino–nucleus interactions and related measurements from electron and pion scattering. We summarize the discussions at the workshop pertaining to the aforementioned issues in quasi-elastic scattering and single photon production, particularly where there was consensus on the highest priority issues to be resolved and the path towards resolving them.

  12. Quasi-elastic and inelastic inclusive electron scattering from an oxygen jet target

    International Nuclear Information System (INIS)

    Anghinolfi, M.; Cenni, R.; Levi Sandri, P.; Longhi, A.; Mokeev, V.I.; Polli, E.; Reolon, A.; Ricco, G.; Simula, S.; Taiuti, M.; Teglia, A.; Zucchiatti, A.

    1996-01-01

    The results of an experiment on inclusive electron scattering from an oxygen jet target, performed in a wide range of energy and momentum transfer covering both quasi-elastic and Δ(1232) resonance regions, are reported. In the former region the theoretical predictions, obtained including effects of nucleon-nucleon correlations in both initial and final states, give a good description of the experimental data. In the inelastic region a broadening as well as a damping of the resonant part of the cross section with respect to the free nucleon case is observed. The need of more detailed calculations including nuclear structure effects on the electroproduction cross section of nucleon resonances is highlighted. (orig.)

  13. Incoherent neutron scattering in acetanilide and three deuterated derivatives

    Science.gov (United States)

    Barthes, Mariette; Almairac, Robert; Sauvajol, Jean-Louis; Moret, Jacques; Currat, Roland; Dianoux, José

    1991-03-01

    Incoherent-neutron-scattering measurements of the vibrational density of states of acetanilide and three deuterated derivatives are presented. These data allow one to identify an intense maximum, assigned to the N-H out-of-plane bending mode. The data display the specific behavior of the methyl torsional modes: large isotopic shift and strong low-temperature intensity; confirm our previous inelastic-neutron-scattering studies, indicating no obvious anomalies in the range of frequency of the acoustic phonons. In addition, the data show the existence of thermally activated quasielastic scattering above 100 K, assigned to the random diffusive motion of the methyl protons. These results are discussed in the light of recent theoretical models proposed to explain the anomalous optical properties of this crystal.

  14. Calculations of neutron spectra after neutron-neutron scattering

    Energy Technology Data Exchange (ETDEWEB)

    Crawford, B E [Gettysburg College, Box 405, Gettysburg, PA 17325 (United States); Stephenson, S L [Gettysburg College, Box 405, Gettysburg, PA 17325 (United States); Howell, C R [Duke University and Triangle Universities Nuclear Laboratory, Durham, NC 27708-0308 (United States); Mitchell, G E [North Carolina State University, Raleigh, NC 27695-8202 (United States); Tornow, W [Duke University and Triangle Universities Nuclear Laboratory, Durham, NC 27708-0308 (United States); Furman, W I [Joint Institute for Nuclear Research, 141980 Dubna (Russian Federation); Lychagin, E V [Joint Institute for Nuclear Research, 141980 Dubna (Russian Federation); Muzichka, A Yu [Joint Institute for Nuclear Research, 141980 Dubna (Russian Federation); Nekhaev, G V [Joint Institute for Nuclear Research, 141980 Dubna (Russian Federation); Strelkov, A V [Joint Institute for Nuclear Research, 141980 Dubna (Russian Federation); Sharapov, E I [Joint Institute for Nuclear Research, 141980 Dubna (Russian Federation); Shvetsov, V N [Joint Institute for Nuclear Research, 141980 Dubna (Russian Federation)

    2004-09-01

    A direct neutron-neutron scattering length, a{sub nn}, measurement with the goal of 3% accuracy (0.5 fm) is under preparation at the aperiodic pulsed reactor YAGUAR. A direct measurement of a{sub nn} will not only help resolve conflicting results of a{sub nn} by indirect means, but also in comparison to the proton-proton scattering length, a{sub pp}, shed light on the charge-symmetry of the nuclear force. We discuss in detail the analysis of the nn-scattering data in terms of a simple analytical expression. We also discuss calibration measurements using the time-of-flight spectra of neutrons scattered on He and Ar gases and the neutron activation technique. In particular, we calculate the neutron velocity and time-of-flight spectra after scattering neutrons on neutrons and after scattering neutrons on He and Ar atoms for the proposed experimental geometry, using a realistic neutron flux spectrum-Maxwellian plus epithermal tail. The shape of the neutron spectrum after scattering is appreciably different from the initial spectrum, due to collisions between thermal-thermal and thermal-epithermal neutrons. At the same time, the integral over the Maxwellian part of the realistic scattering spectrum differs by only about 6 per cent from that of a pure Maxwellian nn-scattering spectrum.

  15. Ratio of spin transfer parameters dt/rt in d(p vector, n vector)pp quasi-elastic scattering

    International Nuclear Information System (INIS)

    Abegg, R.; Green, W.; Greeniaus, L.G.; Miller, C.A.; Bardyopadhyay, D.; Birchall, J.; Davis, C.A.; Davison, N.E.; Page, S.A.; Ramsay, W.D.; van Oers, W.T.H.; Lapointe, C.; Moss, G.A.; Tkachuk, R.R.

    1988-05-01

    The ratio of spin transfer parameters d t /r t for the quasi-elastic process d(p,n)pp has been measured at four energies between 200 and 500 MeV at a neutron scattering angle of 9 degrees. From this, the following values of D t /R t for free np scattering have been deduced: -0.0190 ± 0.0072 (T p = 223 MeV); -0.2328 ± 0.0057 (324 MeV); -0.3731 ± 0.0068 (425 MeV); -0.4892 ± 0.0107 (492 MeV). These values have a noticeable effect on present day phase shift solutions. The magnitude of the ε 1 mixing parameter is reduced and other phase shifts are smoother around 300 MeV. (Author) (17 refs., 2 tabs., 3 figs.)

  16. Theoretical study of the slow neutron coherent scattering by nemanic liquid crystals

    International Nuclear Information System (INIS)

    Sugakov, V.I.; Shiyanovskij, S.V.

    1982-01-01

    An exact expression is obtained for neutron coherent quasielastic scattering cross section in nematic liquid crystals. Expressions are analyzed or big and small values of scattering wave vector. In the first case scattering is occured on the separate molecules and the account of the molecule form noncylindricity is to be essential. In the second case an intermolecular correlations contribute greatly to cross sections. A connection is found for pair correlation function with fluctuation for density, dipole moment and order parameters. The performed cross section analysis allow to determine the significant microscopic parameters of the nematic liquid crystal from the experimental data of slow neutron scattering

  17. Diffusion of water adsorbed in hydrotalcite: neutron scattering Study

    Energy Technology Data Exchange (ETDEWEB)

    Mitra, S [Solid State Physics Division, Bhabha Atomic Research Centre, Mumbai (India); Pramanik, A [Unilever Research India, Bangalore 500 066 (India); Chakrabarty, D [Godrej Sara Lee Limited, Research and Development Centre, Mumbai 400 079 (India); Juranyi, F [Laboratory for Neutron Scattering, ETHZ and PSI, CH-5232 Villigen PSI (Switzerland); Gautam, S [Solid State Physics Division, Bhabha Atomic Research Centre, Mumbai (India); Mukhopadhyay, R [Solid State Physics Division, Bhabha Atomic Research Centre, Mumbai (India)

    2007-12-15

    Layered double hydroxides (LDH) are a class of ionic lamellar solids with positively charged layers of two kinds of metallic cations and exchangeable hydrated anions. Quasi-elastic neutron scattering (QENS) measurements are performed in this type of LDH structured hydrated hydrotalcite sample to study the dynamical behaviour of the water in geometric confinement within the layers. Dynamical parameters correspond to the confined water molecules revealed that depending on the amount of excess water present, behaves differently and approaches bulk values at high concentration. Both translational and rotational dynamical parameters showed that at very low concentration of excess water, water molecules are attached to the surfaces and show the confinement effect.

  18. A study of quasi-elastic muon (anti) neutrino scattering in the NOMAD experiment

    International Nuclear Information System (INIS)

    Lyubushkin, V.V.; Popov, B.A.

    2008-01-01

    We have studied the muon neutrino and antineutrino-quasi-elastic (QEL) scattering reactions (ν μ n → μ - p and νbar μ p → μ + n) using a set of experimental data collected by the NOMAD collaboration. We have performed measurements of the cross section of these processes on a nuclear target (mainly carbon) normalizing it to the total ν μ (νbar μ ) charged current cross section. The results for the flux averaged QEL cross sections in the (anti)neutrino energy interval 3-100 GeV are (σ qel )ν μ = (0.92 ± 0.02 (stat.) ± 0.06 (syst.)) · 10 -38 cm 2 and (σ qel )νbar μ = (0.81 ± 0.05 (stat.) ± 0.08 (syst.)) · 10 -38 cm 2 for neutrino and antineutrino, respectively. The axial mass parameter M A was extracted from the measured quasi-elastic neutrino cross section. The corresponding result is M A = 1.05 ± 0.02 (stat.) ± 0.06 (syst.) GeV. It is consistent with the axial mass values recalculated from the antineutrino cross section and extracted from the pure Q 2 shape analysis of the high purity sample of ν μ quasi-elastic 2-track events, but has smaller systematic error and should be quoted as the main result of this work. The measured M A is found to be in good agreement with the world average value obtained in the previous deuterium filled bubble chamber experiments. These results do not support M A measurements published recently by the K2K and MiniBooNE collaborations, which reported somewhat larger values, which are however compatible with our results within their large errors

  19. Results on Double-polarization Asymmetries in Quasielastic Scattering from Polarized 3He

    Directory of Open Access Journals (Sweden)

    Sulkosky Vincent A.

    2016-01-01

    Full Text Available The 3He nucleus has become extremely important in the investigation of the neutron’s spin structure. When polarized, 3He acts as an effective polarized neutron target and hence facilitates our understanding of the neutron’s internal structure. However, to be used in this manner, our understanding of the internal structure of 3He is of extreme importance. As the precision of experiments has improved, the extraction of polarized neutron information from 3He leads to an ever larger share of the systematic uncertainty for these experiments. In these proceedings, I present a precise measurement of beam-target asymmetries in the He→3(e→ ,e′d${}^3\\overrightarrow {He} (\\vec e,e'd$ and He→3(e→,e′p${}^3\\overrightarrow {He} (\\vec e,e'p$ reactions. The former process is a uniquely sensitive probe of hadron dynamics in 3He and the structure of the underlying electromagnetic currents. The measurements have been performed around the quasi-elastic peak at Q2 = 0.25 (GeV/c2 and 0.35 (GeV/c2 for recoil momenta up to 270 MeV/c. The experimental apparatus, analysis and results were presented together with a comparison to state-of-the art Faddeev calculations.

  20. Applications of thermal neutron scattering

    International Nuclear Information System (INIS)

    Kostorz, G.

    1978-01-01

    Although in the past neutrons have been used quite frequently in the study of condensed matter, a more recent development has lead to applications of thermal neutron scattering in the investigation of more practical rather than purely academic problems. Physicists, chemists, materials scientists, biologists, and others have recognized and demonstrated that neutron scattering techniques can yield supplementary information which, in many cases, could not be obtained with other methods. The paper illustrates the use of neutron scattering in these areas of applied research. No attempt is made to present all the aspects of neutron scattering which can be found in textbooks. From the vast amount of experimental data, only a few examples are presented for the study of structure and atomic arrangement, ''extended'' structure, and dynamic phenomena in substances of current interest in applied research. (author)

  1. Huang diffuse scattering of neutrons

    International Nuclear Information System (INIS)

    Burkel, E.; Guerard, B. v.; Metzger, H.; Peisl, J.

    1979-01-01

    Huang diffuse neutron scattering was measured for the first time on niobium with interstitially dissolved deuterium as well as on MgO after neutron irradiation and Li 7 F after γ-irradiation. With Huang diffuse scattering the strength and symmetry of the distortion field around lattice defects can be determined. Our results clearly demonstrate that this method is feasible with neutrons. The present results are compared with X-ray experiments and the advantages of using neutrons is discussed in some detail. (orig.)

  2. Commercial applications of neutron scattering

    International Nuclear Information System (INIS)

    Hutchings, M.T.

    1993-01-01

    The fact that industry is now willing to pay the full commercial cost for certain neutron scattering experiments aimed at solving its urgent materials - related problems is a true testimony to the usefulness of neutrons as microscopic probes. This paper gives examples of such use of three techniques drawn mainly from our experience at AEA Technology Harwell Laboratory. These are diffraction to measure residual stress, small angle neutron scattering to examine hardening precipitates in ferritic steels brought about by irradiation, and reflectivity to study amorphous diamond layers deposited on silicon. In most cases it is the penetrative power of the neutron which proves to be its best asset for commercial industrial applicaitons. (author)

  3. Precise measurement of the neutron magnetic form factor from quasielastic 3 rvec He(rvec e,e')

    International Nuclear Information System (INIS)

    Gao, H.

    1997-01-01

    Polarized 3 He targets have proven to be a useful tool for studying the electric and magnetic form factors of the neutron, and the spin structure of the neutron. The neutron magnetic form factor at low Q 2 was determined previously at MIT-Bates from the quasielastic 3 rvec He(rvec e, e ' ) process. New experiment was planned at TJNAF to systematically measure the inclusive 3 He quasielastic transverse asymmetry, A T ' , at Q 2 = 0.1 - 0.5 (GeV/c) 2 with high statistical and systematic accuracy. A 2% statistical uncertainty is aimed at all the pro- posed values of Q 2 , and 3% systematic uncertainty for A T ' can be achieved for this experiment. The precise data will constrain theoretical calculations of 3 He quasielastic asymmetry. Furthermore, the neutron magnetic form factor at Q 2 = 0.1 - 0.5 (GeV/c) 2 will be extracted from the measured asymmetries with an overall uncertainty of 2%. Precise measurements of G n M at low Q 2 will resolve the discrepancy among the existing data in the same Q 2 region

  4. Application of hot neutron scattering to the problem of 3d metallic paramagnetism

    International Nuclear Information System (INIS)

    Brown, P.J.; Capellmann, H.; Deportes, J.; Givord, D.; Johnson, S.M.; Ziebeck, K.R.A.

    1984-01-01

    The authors report in this paper on experiments performed in Fe and Ni in their paramagnetic state. Scattering of polarized neutrons with polarization analysis has been used to separate out the magnetic scattering from other sources of scattering. Large quasi-elastic scattering is observed which characterizes ferromagnetic correlations over several inter-atomic distances. The large-Q component of the scattering is fairly small as expected for itinerant electrons in which the energy of magnetic excitations may be of the order of the bandwidth. These should help discriminate between the itinerant and localized models

  5. Bibliography for thermal neutron scattering

    International Nuclear Information System (INIS)

    Sakamoto, M.; Chihara, J.; Nakahara, Y.; Kadotani, H.; Sekiya, T.

    1976-12-01

    It contains bibliographical references to measurements, calculations, reviews and basic studies on thermal neutron scatterings and dynamical properties of condensed matter. About 2,700 documents up to the end of 1975 are covered. (auth.)

  6. Neutron scattering studies in the actinide region

    International Nuclear Information System (INIS)

    Kegel, G.H.R.; Egan, J.J.

    1993-09-01

    This report discusses the following topics: Prompt fission neutron energy spectra for 235 U and 239 Pu; Two-parameter measurement of nuclear lifetimes; ''Black'' neutron detector; Data reduction techniques for neutron scattering experiments; Inelastic neutron scattering studies in 197 Au; Elastic and inelastic scattering studies in 239 Pu; and neutron induced defects in silicon dioxide MOS structures

  7. Dynamics in γ-Fe2O3 nanoparticles studied by time-of-flight polarized neutron scattering

    DEFF Research Database (Denmark)

    Kuhn, L.T.; Lefmann, K.; Klausen, S.N.

    2004-01-01

    The inelastic neutron-scattering signal from magnetic nanoparticles contains information on magnetic dynamics like superparamagnetic relaxation and collective magnetic excitations. Often another, very broad quasi-elastic component is observed in addition. We have studied this quasi-elastic neutron...... signal from 4 nm ferrimagnetic maghemite (gamma-Fe(2)O(3)) particles, and by means of time-of-flight polarised neutron scattering we have identified the source of (most of) this signal to be water adsorbed at the surface of the nanoparticles. A minor part of the signal has its origin in dynamics...

  8. Neutron scattering. Experiment manuals

    International Nuclear Information System (INIS)

    Brueckel, Thomas; Heger, Gernot; Richter, Dieter; Roth, Georg; Zorn, Reiner

    2012-01-01

    The following topics are dealt with: The thermal triple-axis spectrometer PUMA, the high-resolution powder diffractometer SPODI, the hot single-crystal diffractometer HEiDi for structure analysis with neutrons, the backscattering spectrometer SPHERES, the neutron polarization analyzer DNS, the neutron spin-echo spectrometer J-NSE, the small-angle neutron diffractometers KWS-1/-2, the very-small-angle neutron diffractometer with focusing mirror KWS-3, the resonance spin-echo spectrometer RESEDA, the reflectometer TREFF, the time-of-flight spectrometer TOFTOF. (HSI)

  9. Heterodyne quasi-elastic light-scattering instrument for biomedical diagnostics.

    Science.gov (United States)

    Lebedev, A D; Ivanova, M A; Lomakin, A V; Noskin, V A

    1997-10-20

    The heterodyne technique has a number of advantages over the homodyne technique when an accurate characterization of particle-size distribution (PSD) of heterogeneous systems is required. However, there are problems related to acoustic vibrations that make it difficult to take advantage of the heterodyne technique. An instrument developed for quasi-elastic light scattering (QELS) that uses the optical heterodyning principle is described. Vibration-related problems are considerably reduced because of the incorporation of all optical elements into one solid optical block. A real-time correlation analysis of the photocurrent fluctuations is performed by a PC-embedded analog-to-digital converter card with a digital signal processor. Investigation of the PSD in biological fluids for medical diagnostics is presented as a typical application. A diagnostic analysis of the PSD requires a simultaneous processing of a huge number of QELS data. An original statistical algorithm to accomplish this analysis has been developed. Technical specifications of instrumentation for heterodyne QELS measurement are discussed.

  10. Elastic and quasielastic scattering of light nuclei in the theory of multiple scattering

    International Nuclear Information System (INIS)

    Ismatov, E.I.; Kuterbekov, K.A.; Dzhuraev, Sh.Kh.; Ehsaniyazov, Sh.P.; Zholdasova, S.M.

    2005-01-01

    In the work the calculation method for diffraction scattering amplitudes of light nuclei by heavy nuclei is developed. For A 1 A 2 -scattering effects of pair-, three-fold, and four-fold screenings are estimated. It is shown, that in amplitude calculations for A 1 A 2 elastic scattering it is enough come to nothing more than accounting of total screenings in the first order. Analysis of nucleus-nucleus scattering sensitive characteristics to choice of single-particle nuclear densities parametrization is carried out

  11. The Measurement of the Quasi-Elastic Neutrino-Nucleon Scattering Cross Section at the Tevatron

    Energy Technology Data Exchange (ETDEWEB)

    Suwonjandee, Narumon [Cincinnati U.

    2004-01-01

    The quasi-elastic neutrino nucleon cross section measurement has been measured in the low energy region less than 100 Ge V. The data agree well with the model proposed by C. H. Llewellyn Smith. This model predicts that the quasi-elastic cross section should be constant in the high enery region. The NuTeV experiment at Fermilab provides data which allows us to measure the quasi-elastic cross section for both neutrinos and anti-neutrinos at high energy. We find that $\\sigma^{Neucleon}_{qe}(v) = 0.94 \\pm 0.03(stat.) \\pm 0.07(syst.)$, and $\\sigma^{Neucleon}_{qe}(\\bar\

  12. Quasi-elastic scattering an alternative tool for mapping the fusion barriers for heavy-ion induced fusion reaction

    International Nuclear Information System (INIS)

    Behera, B.R.

    2016-01-01

    Heavy element synthesis through heavy-ion induced fusion reaction is an active field in contemporary nuclear physics. Exact knowledge of fusion barrier is one of the essential parameters for planning any experiments for heavy element production. Theoretically there are many models available to predict the exact barrier. Though these models are successful for predicting the fusion of medium mass nuclei, it somehow fails for predicting the exact location of barrier for fusion of heavy nuclei. Experimental determination of barrier for such reactions is required for future experiments for the synthesis of heavy elements. Traditionally fusion barrier is determined taking a double derivative of fusion excitation function. However, such method is difficult in case of fusion of heavy nuclei due to its very low fusion/capture cross section and its experimental complications. Alternatively fusion barrier can be determined by measuring the quasi-elastic cross section at backward angles. This method can be applied for determining the fusion barrier for the fusion of heavy nuclei. Experimental determination of fusion barrier by different methods and comparison of the fusion excitation function and quasi-elastic scattering methods for the determination of fusion barrier are reviewed. At IUAC, New Delhi recently a program has been started for the measurement of fusion barrier through quasi-elastic scattering methods. The experimental facility and the first results of the experiments carried out with this facility are presented. (author)

  13. Observation of Oxygen Frenkel Disorder in Uranium Dioxide above 2000 K by Use of Neutron-Scattering Techniques

    DEFF Research Database (Denmark)

    Clausen, Kurt Nørgaard; Hayes, W.; Macdonald, J E.

    1984-01-01

    Diffraction and coherent diffuse quasielastic scattering of neutrons have been used to investigate Frenkel disorder of the oxygen sublattice in single crystals of stoichiometric UO2. Measurements were made up to 2900 K using a special high-temperature furnace. The results provide the first direct...

  14. Neutron scattering science in Australia

    Energy Technology Data Exchange (ETDEWEB)

    Knott, Robert [Australian Nuclear Science and Technology Organisation, Menai, NSW (Australia)

    1999-10-01

    Neutron scattering science in Australia is making an impact on a number of fields in the scientific and industrial research communities. The unique properties of the neutron are being used to investigate problems in chemistry, materials science, physics, engineering and biology. The reactor HIFAR at the Australian Nuclear Science and Technology Organisation research laboratories is the only neutron source in Australia suitable for neutron scattering science. A suite of instruments provides a wide range of opportunities for the neutron scattering community that extends throughout universities, government and industrial research laboratories. Plans are in progress to replace the present research reactor with a modern multi-purpose research reactor to offer the most advanced neutron scattering facilities. The experimental and analysis equipment associated with a modern research reactor will permit the establishment of a national centre for world class neutron science research focussed on the structure and functioning of materials, industrial irradiations and analyses in support of Australian manufacturing, minerals, petrochemical, pharmaceuticals and information science industries. (author)

  15. Neutron scattering science in Australia

    International Nuclear Information System (INIS)

    Knott, Robert

    1999-01-01

    Neutron scattering science in Australia is making an impact on a number of fields in the scientific and industrial research communities. The unique properties of the neutron are being used to investigate problems in chemistry, materials science, physics, engineering and biology. The reactor HIFAR at the Australian Nuclear Science and Technology Organisation research laboratories is the only neutron source in Australia suitable for neutron scattering science. A suite of instruments provides a wide range of opportunities for the neutron scattering community that extends throughout universities, government and industrial research laboratories. Plans are in progress to replace the present research reactor with a modern multi-purpose research reactor to offer the most advanced neutron scattering facilities. The experimental and analysis equipment associated with a modern research reactor will permit the establishment of a national centre for world class neutron science research focussed on the structure and functioning of materials, industrial irradiations and analyses in support of Australian manufacturing, minerals, petrochemical, pharmaceuticals and information science industries. (author)

  16. New techniques in neutron scattering

    International Nuclear Information System (INIS)

    Hayter, J.B.

    1993-01-01

    New neutron sources being planned, such as the Advanced Neutron Source (ANS) or the European Spallation Source (ESS), will provide an order of magnitude flux increase over what is available today, but neutron scattering will still remain a signal-limited technique. At the same time, the development of new materials, such as polymer and ceramic composites or a variety of complex fluids, will increasingly require neutron-based research. This paper will discuss some of the new techniques which will allow us to make better use of the available neutrons, either through improved instrumentation or through sample manipulation. Discussion will center primarily on unpolarized neutron techniques since polarized neutrons will be the subject of the next paper. (author)

  17. Neutron scattering from fractals

    DEFF Research Database (Denmark)

    Kjems, Jørgen; Freltoft, T.; Richter, D.

    1986-01-01

    The scattering formalism for fractal structures is presented. Volume fractals are exemplified by silica particle clusters formed either from colloidal suspensions or by flame hydrolysis. The determination of the fractional dimensionality through scattering experiments is reviewed, and recent small...

  18. Recent Advances and Open Questions in Neutrino-induced Quasi-elastic Scattering and Single Photon Production

    Energy Technology Data Exchange (ETDEWEB)

    Garvey, G. T. [Los Alamos; Harris, D. A. [Fermilab; Tanaka, H. A. [British Columbia U.; Tayloe, R. [Indiana U.; Zeller, G. P. [Fermilab

    2015-06-15

    The study of neutrino–nucleus interactions has recently seen rapid development with a new generation of accelerator-based neutrino experiments employing medium and heavy nuclear targets for the study of neutrino oscillations. A few unexpected results in the study of quasi-elastic scattering and single photon production have spurred a revisiting of the underlying nuclear physics and connections to electron–nucleus scattering. A thorough understanding and resolution of these issues is essential for future progress in the study of neutrino oscillations.

  19. Diffusion of Hydrogen in the beta-Phase of Pd-H Studied by Small Energy Transfer Neutron Scattering

    Energy Technology Data Exchange (ETDEWEB)

    Nelin, G; Skoeld, K

    1974-07-01

    The diffusion of hydrogen in beta-PdH has been studied by quasielastic neutron scattering. It is shown that the diffusion occurs through jumps between adjacent octahedral interstitial sites. The observed integrated quasielastic intensities cannot be described by a simple Debye-Waller factor. The phase transition from the beta-phase to the alpha-phase has also been studied. No dramatic changes in the scattering patterns were observed. It is concluded that the diffusion mechanism is remarkably similar between the low concentration alpha-phase and the high concentration beta-phase

  20. Phase transitions and neutron scattering

    International Nuclear Information System (INIS)

    Shirane, G.

    1993-01-01

    A review is given of recent advances in neutron scattering studies of solid state physics. I have selected the study of a structural phase transition as the best example to demonstrate the power of neutron scattering techniques. Since energy analysis is relatively easy, the dynamical aspects of a transition can be elucidated by the neutron probe. I shall discuss in some detail current experiments on the 100 K transition in SrTiO 3 , the crystal which has been the paradigm of neutron studies of phase transitions for many years. This new experiment attempts to clarify the relation between the neutron central peak, observed in energy scans, and the two length scales observed in recent x-ray diffraction studies where only scans in momentum space are possible. (author)

  1. Advances in neutron scattering spectroscopy

    International Nuclear Information System (INIS)

    White, J.W.

    1977-01-01

    Some aspects of the application of neutron scattering to problems in polymer science, surface chemistry, and adsorption phenomena, as well as molecular biology, are reviewed. In all these areas, very significant work has been carried out using the medium flux reactors at Harwell, Juelich and Risoe, even without the use of advanced multidetector techniques or of a neutron cold source. A general tendency can also be distinguished in that, for each of these new fields, a distinct preference for colder neutrons rather than thermal neutron beams can be seen. (author)

  2. New Techniques in Neutron Scattering

    DEFF Research Database (Denmark)

    Birk, Jonas Okkels

    potential performance than any existing facility, however in order to use this pulse structure optimally many existing neutron scattering instruments will need to be redesigned. This defense will concentrate on the design and optimization of the inverse time-of-flight cold neutron spectrometer CAMEA......, simulations and prototyping to optimize the instrument and ensure that it will deliver the predicted performance when constructed. During the design a new prismatic analyser concept that can be of interest to many other neutron spectrometers was developed. The design work was compiled into an instrument......Neutron scattering is an important experimental technique in amongst others solid state physics, biophysics, and engineering. This year construction of European Spallation Source (ESS) was commenced in Lund, Sweeden. The facility will use a new long pulsed source principle to obtain higher...

  3. Neutron spectral modulation as a new thermal neutron scattering technique. Pt. 1

    International Nuclear Information System (INIS)

    Ito, Y.; Nishi, M.; Motoya, K.

    1982-01-01

    A thermal neutron scattering technique is presented based on a new idea of labelling each neutron in its spectral position as well as in time through the scattering process. The method makes possible the simultaneous determination of both the accurate dispersion relation and its broadening by utilizing the resolution cancellation property of zero-crossing points in the cross-correlated time spectrum together with the Fourier transform scheme of the neutron spin echo without resorting to the echoing. The channel Fourier transform applied to the present method also makes possible the determination of the accurate direct energy scan profile of the scattering function with a rather broad incident neutron wavelength distribution. Therefore the intensity sacrifice for attaining high accurarcy is minimized. The technique is used with either a polarized or unpolarized beam at the sample position with no precautions against beam depolarization at the sample for the latter case. Relative time accurarcy of the order of 10 -3 to 10 -4 may be obtained for the general dispersion relation and for the quasi-elastic energy transfers using correspondingly the relative incident neutron wavelength spread of 10 to 1% around an incident neutron energy of a few meV. (orig.)

  4. Anti-Neutrino Charged Current Quasi-Elastic Scattering in MINER$\

    Energy Technology Data Exchange (ETDEWEB)

    Chvojka, Jesse John [Univ. of Rochester, NY (United States)

    2012-01-01

    The phenomenon of neutrino oscillation is becoming increasingly understood with results from accelerator-based and reactor-based experiments, but unanswered questions remain. The proper ordering of the neutrino mass eigenstates that compose the neutrino avor eigenstates is not completely known. We have yet to detect CP violation in neutrino mixing, which if present could help explain the asymmetry between matter and anti-matter in the universe. We also have not resolved whether sterile neutrinos, which do not interact in any Standard Model interaction, exist. Accelerator-based experiments appear to be the most promising candidates for resolving these questions; however, the ability of present and future experiments to provide answers is likely to be limited by systematic errors. A significant source of this systematic error comes from limitations in our knowledge of neutrino-nucleus interactions. Errors on cross-sections for such interactions are large, existing data is sometimes contradictory, and knowledge of nuclear effects is incomplete. One type of neutrino interaction of particular interest is charged current quasi-elastic (CCQE) scattering, which yields a final state consisting of a charged lepton and nucleon. This process, which is the dominant interaction near energies of 1 GeV, is of great utility to neutrino oscillation experiments since the incoming neutrino energy and the square of the momentum transferred to the final state nucleon, Q2, can be reconstructed using the final state lepton kinematics. To address the uncertainty in our knowledge of neutrino interactions, many experiments have begun making dedicated measurements. In particular, the MINER A experiment is studying neutrino-nucleus interactions in the few GeV region. MINERvA is a fine-grained, high precision, high statistics neutrino scattering experiment that will greatly improve our understanding of neutrino cross-sections and nuclear effects that affect the final state particles

  5. Material science and neutron scattering

    International Nuclear Information System (INIS)

    1983-01-01

    Neutron scattering experiments complete and extend the condensed matter studies made with X and gamma rays. Then story show a permanent evolution of the instrumentation, methods and experimental techniques to improve the result quality. This is more especially important as neutron sources are weaker than photon and electron sources. Progress in this research domain is due, in most part, to discovery and development of materials for the different measurement device components [fr

  6. Neutron scattering and HPLC study on L-ascorbic acid and its degradation

    Energy Technology Data Exchange (ETDEWEB)

    Bellocco, E. [Department of Organic and Biological Chemistry, University of Messina, Messina (Italy)], E-mail: bellocco@isengard.unime.it; Barreca, D.; Lagana, G.; Leuzzi, U. [Department of Organic and Biological Chemistry, University of Messina, Messina (Italy); Migliardo, F.; Torre, R. La; Galli, G. [Department of Physics, University of Messina, Messina (Italy); Galtieri, A. [Department of Organic and Biological Chemistry, University of Messina, Messina (Italy); Minutoli, L.; Squadrito, F. [Department of Clinical and Experimental Medicine and Pharmacology, University of Messina, Messina (Italy)

    2008-04-18

    The present paper shows a systematic dynamic and kinetic study on L-ascorbic acid and its degradation at high temperature. The neutron scattering study allows, through the behavior of quasi-elastic neutron scattering (QENS) spectra, to characterize the diffusive dynamics of L-ascorbic acid in water mixtures. Ascorbic acid undergoes degradation process at high temperature, but the presence of trehalose in solution markedly avoids ascorbic acid loss enhancing its t{sub 1/2} (half life time), as determined by high performance liquid chromatography (HPLC)

  7. Influence of the effective mass of water molecule on thermal neutron scattering

    International Nuclear Information System (INIS)

    Markovic, M.

    1981-01-01

    The influence of the effective water molecule mass on the thermal neutron scattering on the nucleus of the hydrogen atom has been investigated. Besides the actual water molecule mass (M = 18) the investigations have been carried out with its two effective values (M1 = 16 and M2 = 20). The differential and total cross sections have been calculated for the incident thermal neutron energy E o = 1 eV. Investigation results show different prominence of the quantum effects and for M2 the appearance of peaks in the quasielastic scattering. (author)

  8. Neutron scattering and HPLC study on L-ascorbic acid and its degradation

    International Nuclear Information System (INIS)

    Bellocco, E.; Barreca, D.; Lagana, G.; Leuzzi, U.; Migliardo, F.; Torre, R. La; Galli, G.; Galtieri, A.; Minutoli, L.; Squadrito, F.

    2008-01-01

    The present paper shows a systematic dynamic and kinetic study on L-ascorbic acid and its degradation at high temperature. The neutron scattering study allows, through the behavior of quasi-elastic neutron scattering (QENS) spectra, to characterize the diffusive dynamics of L-ascorbic acid in water mixtures. Ascorbic acid undergoes degradation process at high temperature, but the presence of trehalose in solution markedly avoids ascorbic acid loss enhancing its t 1/2 (half life time), as determined by high performance liquid chromatography (HPLC)

  9. Enzyme hydration, activity and flexibility : A neutron scattering approach

    International Nuclear Information System (INIS)

    Kurkal-Siebert, V.; Finney, J.L.; Daniel, R.M.; Smith, Jeremy C.

    2006-01-01

    Recent measurements have demonstrated enzyme activity at hydrations as low as 3%. The question of whether the hydration-induced enzyme flexibility is important for activity is addressed by performing picosecond dynamic neutron scattering experiments on pig liver esterase powders at various temperatures as well as solutions. At all temperatures and hydrations investigated here, significant quasielastic scattering intensity is found in the protein, indicating the presence of anharmonic, diffusive motion. As the hydration increases a temperature-dependent dynamical transition appears and strengthens involving additional diffusive motion. At low temperature, increasing hydration resulted in lower flexibility of the enzyme. At higher temperatures, systems containing sufficient number of water molecules interacting with the protein exhibit increased flexibility. The implication of these results is that, although the additional hydration-induced diffusive motion and flexibility at high temperatures in the enzyme detected here may be related to increased activity, they are not required for the enzyme to function

  10. Asymptotic neutron scattering laws for anomalously diffusing quantum particles

    Energy Technology Data Exchange (ETDEWEB)

    Kneller, Gerald R. [Centre de Biophysique Moléculaire, CNRS, Rue Charles Sadron, 45071 Orléans (France); Université d’Orléans, Chateau de la Source-Ave. du Parc Floral, 45067 Orléans (France); Synchrotron-SOLEIL, L’Orme de Merisiers, 91192 Gif-sur-Yvette (France)

    2016-07-28

    The paper deals with a model-free approach to the analysis of quasielastic neutron scattering intensities from anomalously diffusing quantum particles. All quantities are inferred from the asymptotic form of their time-dependent mean square displacements which grow ∝t{sup α}, with 0 ≤ α < 2. Confined diffusion (α = 0) is here explicitly included. We discuss in particular the intermediate scattering function for long times and the Fourier spectrum of the velocity autocorrelation function for small frequencies. Quantum effects enter in both cases through the general symmetry properties of quantum time correlation functions. It is shown that the fractional diffusion constant can be expressed by a Green-Kubo type relation involving the real part of the velocity autocorrelation function. The theory is exact in the diffusive regime and at moderate momentum transfers.

  11. Molecular simulation study to examine the possibility of detecting collective motion in protein by inelastic neutron scattering

    International Nuclear Information System (INIS)

    Yasumasa, Joti; Nobuhiro, Go; Akio, Kitao; Nobuhiro, Go

    2003-01-01

    Inelastic and quasielastic neutron scattering gives the information on the dynamics of biological macromolecules. The combination of computer simulation with neutron scattering experiments allows us to characterize a wide range of dynamical phenomena in condensed phase bio-molecular systems. In this work, the dynamic structure factors in (Q,ω)-space were calculated by using the results of bio-molecular simulations. From the simulated inelastic neutron scattering spectra, we discuss the (Q,ω)-range and the resolution of a detector needed to observe function-related protein dynamics. (authors)

  12. Morphology, surface roughness, electron inelastic and quasi-elastic scattering in elastic peak electron spectroscopy of polymers

    International Nuclear Information System (INIS)

    Lesiak, B.; Kosinski, A.; Nowakowski, R.; Koever, L.; Toth, J.; Varga, D.; Cserny, I.; Sulyok, A.; Gergely, G.

    2006-01-01

    Complete text of publication follows. Elastic peak electron spectroscopy (EPES) deals with the interaction of electrons with atoms of a solid surface, studying the distribution of electrons backscattered elastically. The nearest vicinity of the elastic peak, (low kinetic energy region) reflects both, electron inelastic and quasi-elastic processes. The incident electrons produce surface excitations, inducing surface plasmons with the corresponding loss peaks separated by 1 - 20 eV energy from the elastic peak. Quasi-elastic losses result from the recoil of scattering atoms of different atomic number, Z. The respective energy shift and Doppler broadening of the elastic peak depend on Z, the primary electron energy, E, and the measurement geometry. Quantitative surface analytical application of EPES, such as determination of parameters describing electron transport, requires a comparison of experimental data with corresponding data derived from Monte Carlo (MC) simulation. Several problems occur in EPES studies of polymers. The intensity of elastic peak, considered in quantitative surface analysis, is influenced by both, the inelastic and quasi-elastic scattering processes (especially for hydrogen scattering atoms and primary electron energy above 1000 eV). An additional factor affecting the elastic peak intensity is the surface morphology and roughness. The present work compares the effect of these factors on the elastic peak intensity for selected polymers (polyethylene, polyaniline and polythiophenes). X-ray photoelectron spectroscopy (XPS) and helium pycnometry are applied for deriving the surface atomic composition and the bulk density, while scanning electron microscopy (SEM) and atomic force microscopy (AFM) for determining surface morphology and roughness. According to presented results, the influence of surface morphology and roughness is larger than those of surface excitations or recoil of hydrogen atoms. The component due to recoil of hydrogen atoms can be

  13. Breakup coupling effects on near-barrier quasi-elastic scattering of 6,7Li on 144Sm

    International Nuclear Information System (INIS)

    Otomar, D. R.; Lubian, J.; Gomes, P. R. S.; Monteiro, D. S.; Capurro, O. A.; Arazi, A.; Figueira, J. M.; Marti, G. V.; Heimann, D. Martinez; Negri, A. E.; Pacheco, A. J.; Niello, J. O. Fernandez; Guimaraes, V.; Chamon, L. C.

    2009-01-01

    Excitation functions of quasi-elastic scattering at backward angles have been measured for the 6,7 Li+ 144 Sm systems at near-barrier energies, and fusion barrier distributions have been extracted from the first derivatives of the experimental cross sections with respect to the bombarding energies. The data have been analyzed in the framework of continuum discretized coupled-channel calculations, and the results have been obtained in terms of the influence exerted by the inclusion of different reaction channels, with emphasis on the role played by the projectile breakup.

  14. Effect of the strange axial form factor on structure functions for neutral current neutrino scattering in the quasielastic region

    International Nuclear Information System (INIS)

    Kim, Kyungsik

    2011-01-01

    We study the effect of the strange axial form factor on various structure functions for the neutral reaction of neutrino-nucleus scattering in the quasielastic region within the framework of a relativistic single particle model. We use 12 C as the target nucleus, and the incident neutrino energy range is between 150 MeV and 1.5 GeV. The structure functions are extracted at a fixed three momentum transfer and energy transfer by using the intrinsic helicity of neutrino. While the effect of the strange axial form factor is very small, the effect on various structure functions is exhibited explicitly.

  15. (Quasi)Elastic Electron-Muon Large-Angle Scattering to a Two-Loop Approximation: Vertex Contributions

    CERN Document Server

    Bytev, V V; Shaikhatdenov, B G

    2002-01-01

    We consider a process of quasielastic e\\mu large-angle scattering at high energies with radiative corrections up to a two-loop level. The lowest order radiative correction arising both from one-loop virtual photon emission and a real soft emission are presented to a power accuracy. Two-loop level corrections are supposed to be of three gauge-invariant classes. One of them, so-called vertex contribution, is given in logarithmic approximation. Relation with the renormalization group approach is discussed.

  16. (Quasi)Elastic Electron-Muon Large-Angle Scattering to a Two-Loop Approximation Vertex Contributions

    CERN Document Server

    Bytev, V V; Shaikhatdenov, B G

    2002-01-01

    We consider a process of quasielastic e\\mu large-angle scattering at high energies with radiative corrections up to a two-loop level. The lowest order radiative correction arising both from one-loop virtual photon emission and a real soft emission are presented to a power accuracy. Two-loop level corrections are supposed to be of three gauge-invariant classes. One of them, so-called vertex contribution, is given in logarithmic approximation. Relation with the renormalization group approach is discussed.

  17. Study of the Quasi-Elastic Scattering in the NOvA Detector Prototype

    Energy Technology Data Exchange (ETDEWEB)

    Betancourt, Minerba [Univ. of Minnesota, Minneapolis, MN (United States)

    2013-06-01

    NOvA is a 810 km long base-line neutrino oscillation experiment with two detectors (far 14 KTon and near detector 300 Ton) currently being installed in the NUMI o -axis neutrino beam produced at Fermilab. A 222 Ton prototype NOvA detector (NDOS) was built and operated in the neutrino beam for over a year to understand the response of the detector and its construction. The goal of this thesis is to study the muon neutrino interaction data collected in this test, specifically the identification of quasi-elastic charged-current interactions and measure the behavior of the quasi-elastic muon neutrino cross section.

  18. Theoretical challenges in neutron scattering

    International Nuclear Information System (INIS)

    Lovesey, S.W.

    1985-07-01

    Topics in the interpretation of neutron scattering experiments from paramagnets and quantum fluids are used to illustrate the puissance of the technique in condensed matter research, and to record some fundamental shortcomings in the available theory of many-particle systems. (author)

  19. Bibliography for thermal neutron scattering

    International Nuclear Information System (INIS)

    Sakamoto, Masanobu; Chihara, Junzo; Gotoh, Yorio; Kadotani, Hiroyuki; Sekiya, Tamotsu.

    1979-09-01

    Bibliographic references are given for measurements, calculations, reviews and basic studies of thermal neutron scattering and dynamical properties of condensed matter. This is the sixth edition covering 3,326 articles collected up to 1978. The edition being the final issue of the present bibliography series, a forthcoming edition will be published in a new form of bibliography. (author)

  20. Recent development in magnetic neutron scattering studies

    International Nuclear Information System (INIS)

    Endoh, Yasuo

    1993-01-01

    Neutron scattering results contain many new concepts in modern magnetism. We review here the most recent neutron magnetic scattering studies from so called '214' copper oxide lamellar materials, because a number of important developments in magnetism are condensed in this novel subject. We show that neutron scattering has played crucial role in our understanding of modern magnetism. (author)

  1. Neutron diffuse scattering in magnetite due to molecular polarons

    International Nuclear Information System (INIS)

    Yamada, Y.; Wakabayashi, N.; Nicklow, R.M.

    1980-01-01

    A detailed neutron diffuse scattering study has been carried out in order to verify a model which describes the property of valence fluctuations in magnetite above T/sub V/. This model assumes the existence of a complex which is composed of two excess electrons and a local displacement mode of oxygens within the fcc primitive cell. The complex is called a molecular polaron. It is assumed that at sufficiently high temperatures there is a random distribution of molecular polarons, which are fluctuating independently by making hopping motions through the crystal or by dissociating into smaller polarons. The lifetime of each molecular polaron is assumed to be long enough to induce an instantaneous strain field around it. Based on this model, the neutron diffuse scattering cross section due to randomly distributed dressed molecular polarons has been calculated. A precise measurement of the quasielastic scattering of neutrons has been carried out at 150 K. The observed results definitely show the characteristics which are predicted by the model calculation and, thus, give evidence for the existence of the proposed molecular polarons. From this standpoint, the Verwey transition of magnetite may be viewed as the cooperative ordering process of dressed molecular polarons. Possible extensions of the model to describe the ordering and the dynamical behavior of the molecular polarons are discussed

  2. Some neutron scattering studies on magnetic and molecular phase transitions

    International Nuclear Information System (INIS)

    Bevaart, L.

    1978-01-01

    In this thesis neutron-scattering investigations on two different systems are described. The first study is concerned with the magnetic ordering phenomena in pseudo two-dimensional (d = 2), two-component antiferromagnets K 2 Mnsub(1-x)Msub(x)F 4 (M = Fe, Co), as a function of the composition x and temperature T. For one of the samples in this series, K 2 Musub(0.978)Fesub(0.022)F 4 , the influence of an external magnetic field on the ordering characteristics was studied in addition. The second study deals with the rotational motions of the NH 4 + groups in NH 4 ZnF 3 in relation with the structural phase transition at Tsub(c) = 115.1 K. The experimental techniques were chosen according to the requirements of each of these two subjects. The former study was carried out by observing the elastic magnetic neutron scattering with a double-axis diffractometer, whereas for the latter study time-of-flight (TOF) techniques were applied to observe the inelastic and quasi-elastic incoherent neutron scattering by the protons of the rotating NH 4 + groups. (Auth.)

  3. Nuclear effects in (anti)neutrino charge-current quasielastic scattering at MINER νA kinematics

    Science.gov (United States)

    Ivanov, M. V.; Antonov, A. N.; Megias, G. D.; González-Jiménez, R.; Barbaro, M. B.; Caballero, J. A.; Donnelly, T. W.; Udías, J. M.

    2018-05-01

    We compare the characteristics of the charged-current quasielastic (anti)neutrino scattering obtained in two different nuclear models, the phenomenological SuperScaling Approximation and the model using a realistic spectral function S(p, ɛ) that gives a scaling function in accordance with the (e, e‧ ) scattering data, with the recent data published by the MiniBooNE, MINER νA, and NOMAD collaborations. The spectral function accounts for the nucleon-nucleon (NN) correlations by using natural orbitals from the Jastrow correlation method and has a realistic energy dependence. Both models provide a good description of the MINER νA and NOMAD data without the need of an ad hoc increase of the value of the mass parameter in the axial-vector dipole form factor. The models considered in this work, based on the the impulse approximation (IA), underpredict the MiniBooNE data for the flux-averaged charged-current quasielastic {ν }μ ({\\bar{ν }}μ ){+}12\\text{C} differential cross section per nucleon and the total cross sections, although the shape of the cross sections is represented by the approaches. The discrepancy is most likely due to missing of the effects beyond the IA, e.g., those of the 2p–2h meson exchange currents that have contribution in the transverse responses.

  4. Interface detection by neutron scattering

    International Nuclear Information System (INIS)

    De Monchy, A.R.; Kok, C.A.; Dorrepaal, J.

    1979-01-01

    A method and apparatus for detecting an interface of materials having different hydrogen content present in a metal vessel or pipe eg. made of steel, are described. Steel walls of columns, reactors, pipelines etc can be monitored. It is very suitable for detection of liquid water or hydrocarbons present in gas pipelines and also for the detection of a liquid hydrocarbon in a vessel or column. A series of measurements of the hydrogen density of the contents of a vessel or pipe are made using at least one californium-252 neutron source located near the outer side of the pipe. Neutrons are emitted and are scattered by the contents of the pipe. At least one neutron detector is located near the outer side of the metal wall. The detectors have a higher sensitivity for scattered neutrons (from the light hydrogen nuclei present in water or hydrocarbons). A source of 0.1 - 1 micrograms produces enough neutrons for most technical applications so the handling is relatively safe although shielding is advocated. The detectors contain helium-3 at a pressure of about 10 bar. Current pulses from the detector are counted. (U.K.)

  5. Detection of explosives by neutron scattering

    International Nuclear Information System (INIS)

    Brooks, F.D.; Buffler, A.; Allie, M.S.; Nchodu, M.R.; Bharuth-Ram, K.

    1998-01-01

    For non-intrusive detection of hidden explosives or other contraband such as narcotics a fast neutron scattering analysis (FNSA) technique is proposed. An experimental arrangement uses a collimated, pulsed beam of neutrons directed at the sample. Scattered neutrons are detected by liquid scintillation counters at different scattering angles. A scattering signature is derived from two-parameter data, counts vs pulse height and time-of-flight measured for each element (H, C, N or O) at each of two scattering angles and two neutron energies. The elemental signatures are very distinctive and constitute a good response matrix for unfolding elemental components from the scattering signatures measured for different compounds

  6. Summary of neutron scattering lengths

    International Nuclear Information System (INIS)

    Koester, L.

    1981-12-01

    All available neutron-nuclei scattering lengths are collected together with their error bars in a uniform way. Bound scattering lengths are given for the elements, the isotopes, and the various spin-states. They are discussed in the sense of their use as basic parameters for many investigations in the field of nuclear and solid state physics. The data bank is available on magnetic tape, too. Recommended values and a map of these data serve for an uncomplicated use of these quantities. (orig.)

  7. Inelastic neutron scattering from clusters

    International Nuclear Information System (INIS)

    Gudel, H.U.

    1985-01-01

    Magnetic excitations in clusters of paramagnetic ions have non-vanishing cross-sections for inelastic neutron scattering (INS). Exchange splittings can be determined, the temperature dependence of exchange can be studied, intra- and intercluster effects can be separated and magnetic form factors determined. INS provides a more direct access to the molecular properties than bulk techniques. Its application is restricted to complexes with no or few (< 10%) hydrogen atoms

  8. Polymer research by neutron scattering

    International Nuclear Information System (INIS)

    Richter, D.

    1993-01-01

    Polymer physics aims on an understanding of the macroscopic behavior of polymer systems on the basis of their molecular structure and dynamics. For this purpose neutrons serve as a unique probe, allowing a simultaneous investigation of polymer structure and dynamics on a molecular scale. Furthermore, hydrogen deuterium exchange facilitates molecular labeling and offers the possibility to observe selected chains or chain parts in dense systems. Neutron small angle scattering reveals information on the conformation and possible aggregation of polymer chains. Data on linear and star like molecules are shown as examples. High resolution neutron spin-echospectroscopy observes the molecular dynamics of long chain molecules. Results on the large scale motion of chins in polymer melts are presented. finally, experiments on chain relaxation close to the glass transition are displayed. Three distinctly different relaxation processes are revealed. (author)

  9. Scattering of Neutrons on Fluctuations of the Density of the Thin Films

    Directory of Open Access Journals (Sweden)

    S. G. ABDULVAHABOVA

    2016-11-01

    Full Text Available Abstract. The cross section for scattering neutron  on the density of  fluctuations of the  thin films is obtained in the framework of the quantum theory of multiple scattering  in the quasielastic approximation. Inhomogeneity can be caused by dynamic density fluctuations, and be statistical in nature. Fluctuations in the density of the scattering material cause neutron scattering wave. The probability of a collision between a neutron and an atomic nucleus depends on the number of neutrons and on their velocity. The formulas have been obtained under the assumption that the imaginary part of the optical potential is a local operator. It was determined that the scattering in density fluctuations does not contribute to the attenuation of the coherent neutron wave. In the approximation of a thin target the solution of the equation for the total scattering amplitude is identical to the expression obtained in the usual eikonal approximation and differs significantly, at least functionally, from the solution for the case of a thick target. There have been detailed investigations of the reflection and refraction of neutron waves in matter, and the details of their dispersion law have been studied. The results are  hown  also, that  the total cross section for scattering by the complete target becomes universal and does not depend on cross section for scattering by one nucleus.Keywords: 25.40-Ep

  10. Neutron scattering and models: Silver

    International Nuclear Information System (INIS)

    Smith, A.B.

    1996-07-01

    Differential neutron elastic-scattering cross sections of elemental silver were measured from 1.5 → 10 MeV at ∼ 100 keV intervals up to 3 MeV, at ∼ 200 keV intervals from 3 → 4 MeV, and at ∼ 500 keV intervals above 4 MeV. At ≤ 4 MeV the angular range of the measurements was ∼ 20 0 → 160 0 with 10 measured values below 3 MeV and 20 from 3 → 4 MeV at each incident energy. Above 4 MeV ≥ 40 scattering angles were used distributed between ∼ 17 0 and 16 0 All of the measured elastic distributions included some contributions due to inelastic scattering. Below 4 MeV the measurements determined cross sections for ten inelastically-scattered neutron groups corresponding to observed excitations of 328 ± 13, 419 ± 50, 748 ± 25, 908 ± 26, 115 ± 38, 1286 ± 25, 1507 ± 20, 1632 ± 30, 1835 ± 20 and 1944 ± 26 keV. All of these inelastic groups probably were composites of contributions from the two isotopes 107 Ag and 109 Ag. The experimental results were interpreted in terms of the spherical optical model and of rotational and vibrational coupled-channels models, and physical implications are discussed. In particular, the neutron-scattering results are consistent with a ground-state rotational band with a quadrupole deformation Β 2 = 0.20 ± ∼ 10% for both of the naturally-occurring silver isotopes

  11. Quasi-elastic cross sections for 1GeV proton incident on {sup 4}He and {sup 12}C

    Energy Technology Data Exchange (ETDEWEB)

    Nishimura, M.; Nakamoto, T.; Shigyo, N. [Kyushu Univ., Fukuoka (Japan). Faculty of Engineering] [and others

    1997-03-01

    The experiment of p-n quasi-elastic scattering cross sections was carried out for 1GeV protons on {sup 4}He and {sup 12}C. The coincident measurement was made at c.m. angles of {+-} 90deg. The experiment was simulated by the use of HETC (High Energy Transport Code). It was examined to apply the p-n quasi-elastic scattering cross sections to neutron flux measurement. (author)

  12. Secondary relaxation in two engineering thermoplastics by neutron scattering and dielectric spectroscopy

    CERN Document Server

    Arrese, S; Alegria, A; Colmenero, J; Frick, B

    2002-01-01

    We present a preliminary investigation of the dynamics of glassy polycarbonate (PC) and polysulfone (PSF) by means of quasielastic neutron scattering and dielectric spectroscopy. Whereas the consideration of pure phenylene ring pi-flips is enough to explain the momentum-transfer (Q) dependence of the inelastic intensity measured for PSF, in the case of PC the Q dependence of both the coherent and the incoherent scattering functions reveal the existence in this polymer of some more complex motion of the phenylene ring. On the other hand, the similarity of the energy landscapes deduced from the different techniques points to a closely related molecular origin for all the relaxation/motions observed. (orig.)

  13. Secondary relaxation in two engineering thermoplastics by neutron scattering and dielectric spectroscopy

    International Nuclear Information System (INIS)

    Arrese-Igor, S.; Arbe, A.; Alegria, A.; Colmenero, J.; Frick, B.

    2002-01-01

    We present a preliminary investigation of the dynamics of glassy polycarbonate (PC) and polysulfone (PSF) by means of quasielastic neutron scattering and dielectric spectroscopy. Whereas the consideration of pure phenylene ring π-flips is enough to explain the momentum-transfer (Q) dependence of the inelastic intensity measured for PSF, in the case of PC the Q dependence of both the coherent and the incoherent scattering functions reveal the existence in this polymer of some more complex motion of the phenylene ring. On the other hand, the similarity of the energy landscapes deduced from the different techniques points to a closely related molecular origin for all the relaxation/motions observed. (orig.)

  14. Neutron scattering lengths of 3He

    International Nuclear Information System (INIS)

    Alfimenkov, V.P.; Akopian, G.G.; Wierzbicki, J.; Govorov, A.M.; Pikelner, L.B.; Sharapov, E.I.

    1976-01-01

    The total neutron scattering cross-section of 3 He has been measured in the neutron energy range from 20 meV to 2 eV. Together with the known value of coherent scattering amplitude it leads to the two sts of n 3 He scattering lengths

  15. Final-state interactions and superscaling in the semi-relativistic approach to quasielastic electron and neutrino scattering

    International Nuclear Information System (INIS)

    Amaro, J. E.; Barbaro, M. B.; Caballero, J. A.; Donnelly, T. W.; Udias, J. M.

    2007-01-01

    The semi-relativistic approach to electron and neutrino quasielastic scattering from nuclei is extended to include final-state interactions. Starting with the usual nonrelativistic continuum shell model, the problem is relativized by using the semi-relativistic expansion of the current in powers of the initial nucleon momentum and relativistic kinematics. Two different approaches are considered for the final-state interactions: the Smith-Wambach 2p-2h damping model and the Dirac-equation-based potential extracted from a relativistic mean-field plus the Darwin factor. Using the latter, the scaling properties of (e,e ' ) and (ν μ ,μ - ) cross sections for intermediate momentum transfers are investigated

  16. Instruments and accessories for neutron scattering research

    International Nuclear Information System (INIS)

    Ishii, Yoshinobu; Morii, Yukio

    2000-04-01

    This report describes neutron scattering instruments and accessories installed by four neutron scattering research groups at the ASRC (Advanced Science Research Center) of the JAERI and the recent topics of neutron scattering research using these instruments. The specifications of nine instruments (HRPD, BIX-I, TAS-1 and PNO in the reactor hall, RESA, BIX-II, TAS-2, LTAS and SANS-J in the guide hall of the JRR-3M) are summarized in this booklet. (author)

  17. Current status of neutron scattering in Thailand

    International Nuclear Information System (INIS)

    Ampornrat, Pantip

    1999-01-01

    Thailand's neutron spectrometer has been installed soon after the startup of the reactor. The neutron scattering experiments have been done continuously, although there were some problems involving the neutron intensity and instruments. Development program has been planned for better experimental result. This paper reports the past and present status of neutron scattering equipment and experiments in Thailand. In addition, installation of a HRPD (High Resolution Powder Diffraction) system is included within the scope of the Ongkharak Nuclear Research Center project. (author)

  18. Neutron scattering studies in the actinide region

    International Nuclear Information System (INIS)

    Beghian, L.E.; Kegel, G.H.R.

    1991-08-01

    During the report period we have investigated the following areas: Neutron elastic and inelastic scattering measurements on 14 N, 181 Ta, 232 Th, 238 U and 239 Pu; Prompt fission spectra for 232 Th, 235 U, 238 U and 239 Pu; Theoretical studies of neutron scattering; Neutron filters; New detector systems; and Upgrading of neutron target assembly, data acquisition system, and accelerator/beam-line apparatus

  19. Neutron scattering studies of the dynamics of biological systems as a function of hydration, temperature and pressure

    International Nuclear Information System (INIS)

    Trapp, Marcus

    2010-01-01

    Incoherent elastic and quasi-elastic neutron scattering were used to measure membrane and protein dynamics in the nano- to picosecond time and Angstrom length scale. The hydration dependent dynamics of DMPC model membranes was studied using elastic and quasi-elastic neutron scattering. The elastic experiments showed a clear shift of the temperature of the main phase transition to higher temperatures with decreasing hydration level. The performed quasi-elastic measurements demonstrated nicely the influence, hydration has on the diffusive motions of the head lipid groups. Different models are necessary to fit the Q-dependence of the elastic incoherent structure factor and show therefore the reduced mobility as a result of reduced water content. In addition to temperature, pressure as a second thermodynamic variable was used to explore dynamics of DMPC membranes. The ordering introduced by applying pressure has similar effect to decreased hydration, therefore both approaches are complementary. Covering three orders of magnitude in observation time, the dynamics of native AChE and its complexed counterpart in presence of Huperzin A was investigated in the range from 1 ns to 100 ps. The mean square displacements obtained from the elastic data allowed the determination of activation energies and gave evidence that a hierarchy of motions contributes to the enzymatic activity. Diffusion constants and residence times were extracted from the quasi-elastic broadening. (author) [fr

  20. Inclusive electron scattering from nuclei in the quasielastic region at large momentum transfer

    Energy Technology Data Exchange (ETDEWEB)

    Fomin, Nadia [California Inst. of Technology (CalTech), Pasadena, CA (United States)

    2008-12-01

    Experiment E02-019, performed in Hall C at the Thomas Jefferson National Accelerator Facility (TJNAF), was a measurement of inclusive electron cross sections for several nuclei (2H,3He, 4He, 9Be,12C, 63Cu, and 197Au) in the quasielastic region at high momentum transfer. In the region of low energy transfer, the cross sections were analyzed in terms of the reduced response, F(y), by examining its y-scaling behavior. The data were also examined in terms of the nuclear structure function νWA 2 and its behavior in x and the Nachtmann variable ξ. The data show approximate scaling of νWA 2 in ξ for all targets at all kinematics, unlike scaling in x, which is confined to the DIS regime. However, y-scaling observations are limited to the kinematic region dominated by the quasielastic response (y <0), where some scaling violations arising from FSIs are observed.

  1. Thermal neutron scattering from a hydrogen-metal system in terms of a general multi-sublattice jump diffusion model

    International Nuclear Information System (INIS)

    Kutner, R.; Sosnowska, I.

    1977-01-01

    A Multi-Sublattice Jump Diffusion Model (MSJD) for hydrogen diffusion through interstitial-site lattices is presented. The MSJD approach may, in principle, be considered as an extension of the Rowe et al (J. Phys. Chem. Solids; 32:41 (1971)) model. Jump diffusion to any neighbours with different jump times which may be asymmetric in space is discussed. On the basis of the model a new method of calculating the diffusion tensor is advanced. The quasielastic, double differential cross section for thermal neutron scattering is obtained in terms of the MSJD model. The model can be used for systems in which interstitial jump diffusion of impurity particles occurs. In Part II the theoretical results are compared with those for quasielastic neutron scattering from the αNbHsub(x) system. (author)

  2. Dynamics in poly vinyl alcohol (PVA) based hydrogel: Neutron scattering study

    Energy Technology Data Exchange (ETDEWEB)

    Prabhudesai, S. A., E-mail: swapnil@barc.gov.in; Mitra, S.; Mukhopadhyay, R. [Solid State Physics Division, Bhabha Atomic Research Centre, Mumbai 40085 (India); Lawrence, Mathias B. [Department of Physics, St. Xavier’s College, Mapusa, Goa 403507 (India); Desa, J. A. E. [Department of Physics, Goa University, Taleigao Plateau, Goa 403206 (India)

    2015-06-24

    Results of quasielastic neutron scattering measurements carried out on Poly Vinyl Alcohol (PVA) based hydrogels are reported here. PVA hydrogels are formed using Borax as a cross-linking agent in D{sub 2}O solvent. This synthetic polymer can be used for obtaining the hydrogels with potential use in the field of biomaterials. The aim of this paper is to study the dynamics of polymer chain in the hydrogel since it is known that polymer mobility influences the kinetics of loading and release of drugs. It is found that the dynamics of hydrogen atoms in the polymer chain could be described by a model where the diffusion of hydrogen atoms is limited within a spherical volume of radius 3.3 Å. Average diffusivity estimated from the behavior of quasielastic width is found to be 1.2 × 10{sup −5} cm{sup 2}/sec.

  3. Neutron scattering measurements from cryogenic ammonia: a progress report

    International Nuclear Information System (INIS)

    Carpenter, J.; Micklich, B.; Zanotti, J.M.

    2004-01-01

    We survey the results of an earlier study of the inelastic scattering from solid ammonia, and report the results of a preliminary experiment carried out at the ∝100 μeV-resolution quasielastic scattering spectrometer QENS at IPNS. (orig.)

  4. Lectures on neutron scattering techniques: 1

    International Nuclear Information System (INIS)

    Carlile, C.J.

    1988-08-01

    The lecture on the production of neutrons was presented at a Summer School on neutron scattering, Rome, 1986. A description is given of the production of neutrons by natural radioactive sources, fission, and particle accelerator sources. Modern neutron sources with high intensities are discussed including the ISIS pulsed neutron source at the Rutherford Appleton Laboratory and the High Flux Reactor at the Institut Laue Langevin. (U.K.)

  5. Structure and dynamics of nonaqueous electrolyte solutions by small angle neutron scattering, brownian dynamics and primitive model theories

    International Nuclear Information System (INIS)

    Kunz, W.; Turq, P.

    1990-01-01

    The study of electrolyte solutions by small angle neutron scattering (static) of quasi-elastic neutron scattering (dynamics) gives new perspectives to the primitive model of electrolytes, for both static and dynamic properties of those systems. Whereas all properties can be interpreted by brownian dynamics, integral equations cannot be used at the present time to get transport coefficients in all cases. As regards the choice of the potentials at the McMillan Mayer level, specific Gurney terms for solvation are not needed for tetraalkylammonium salts. (orig.)

  6. Application of neutron scattering in polymers

    International Nuclear Information System (INIS)

    Han, C.C.

    2003-01-01

    Full text: Neutron scattering offers many opportunities in sciences and technology. This is particularly true in the field of polymer sciences and materials. It is mainly because that the scattering length scales (q -1 ) and scattering contrast (scattering cross-sections) makes neutron a perfect tool for polymer studies. Several examples will be used to illustrate the importance of the small angle neutron scattering and the neutron reflection studies in polymer physics. These include the determination of phase diagram, interaction parameter, and spinodal decomposition kinetics by SANS. In the dynamics area, examples will be given to illustrate the critical temperature shift and mixing of polymer blends under shear flow. Also, the confinement effect on the phase separated structure of polymer blend films will be used to demonstrate the importance of the neutron reflectivity measurement

  7. American Conference on Neutron Scattering 2014

    International Nuclear Information System (INIS)

    Dillen, J. Ardie

    2014-01-01

    Scientists from the around the world converged in Knoxville, TN to have share ideas, present technical information and contribute to the advancement of neutron scattering. Featuring over 400 oral/poster presentations, ACNS 2014 offered a strong program of plenary, invited and contributed talks and poster sessions covering topics in soft condensed matter, hard condensed matter, biology, chemistry, energy and engineering applications in neutron physics - confirming the great diversity of science that is enabled by neutron scattering.

  8. Inelastic neutron scattering from superconducting rings

    International Nuclear Information System (INIS)

    Agafonov, A.I.

    2010-01-01

    For the first time the differential cross section for the inelastic magnetic neutron scattering by superconducting rings is derived taking account of the interaction of the neutron magnetic moment with the magnetic field generated by the superconducting current. Calculations of the scattering cross section are carried out for cold neutrons and thin film rings from type-II superconductors with the magnetic fields not exceeding the first critical field.

  9. American Conference on Neutron Scattering 2014

    Energy Technology Data Exchange (ETDEWEB)

    Dillen, J. Ardie [Materials Research Society, Warrendale, PA (United States)

    2014-12-31

    Scientists from the around the world converged in Knoxville, TN to have share ideas, present technical information and contribute to the advancement of neutron scattering. Featuring over 400 oral/poster presentations, ACNS 2014 offered a strong program of plenary, invited and contributed talks and poster sessions covering topics in soft condensed matter, hard condensed matter, biology, chemistry, energy and engineering applications in neutron physics – confirming the great diversity of science that is enabled by neutron scattering.

  10. Neutron scattering and models: molybdenum

    International Nuclear Information System (INIS)

    Smith, A.B.

    1999-01-01

    A comprehensive interpretation of the fast-neutron interaction with elemental and isotopic molybdenum at energies of le 30 MeV is given. New experimental elemental-scattering information over the incident energy range 4.5 r a rrow 10 MeV is presented. Spherical, vibrational and dispersive models are deduced and discussed, including isospin, energy-dependent and mass effects. The vibrational models are consistent with the ''Lane potential''. The importance of dispersion effects is noted. Dichotomies that exist in the literature are removed. The models are vehicles for fundamental physical investigations and for the provision of data for applied purposes. A ''regional'' molybdenum model is proposed. Finally, recommendations for future work are made

  11. Neutron scattering equipments in JAERI. Current status

    International Nuclear Information System (INIS)

    Hamaguchi, Yoshikazu; Minakawa, Nobuaki

    2003-01-01

    24 neutron scattering instruments are installed in the JRR-3M research reactor. Among them JAERI has 12 neutron scattering instruments. Those instruments are HRPD for high-resolution structural analysis, TAS-1 and TAS-2 for elastic and inelastic scattering and for magnetic scattering measurements by the polarized neutron, LTAS for elastic and inelastic scattering measurement at a low energy region, and for neutron device development, PNO for topography and for very small angle scattering measurement in a small Q range, NRG for neutron radiography, RESA for internal strain measurements, SANS for the molecule and semi-macroscopic magnetic structural analysis, BIX-2 and BIX-3 for the biological structural analysis research, and PGA for the research of prompt gamma-ray analysis. The university groups have 12 neutron scattering instruments. Since those instruments were installed at the period when JRR-3M was completed, about 10 years have passed. In order to match the old control systems with the progress of recent computer technologies, and peripheral equipment, numbers of instruments are being renewed. In the neutron guide hall of JRR-3M, the Ni mirror guide tube was replaced by a super mirror guide tube to increase neutron flux. The intensity of 2A flux was increased by a factor of about two. (J.P.N.)

  12. Synchrotron radiation-based quasi-elastic scattering using time-domain interferometry with multi-line gamma rays.

    Science.gov (United States)

    Saito, Makina; Masuda, Ryo; Yoda, Yoshitaka; Seto, Makoto

    2017-10-02

    We developed a multi-line time-domain interferometry (TDI) system using 14.4 keV Mössbauer gamma rays with natural energy widths of 4.66 neV from 57 Fe nuclei excited using synchrotron radiation. Electron density fluctuations can be detected at unique lengths ranging from 0.1 nm to a few nm on time scales from several nanoseconds to the sub-microsecond order by quasi-elastic gamma-ray scattering (QGS) experiments using multi-line TDI. In this report, we generalize the established expression for a time spectrum measured using an identical single-line gamma-ray emitter pair to the case of a nonidentical pair of multi-line gamma-ray emitters by considering the finite energy width of the incident synchrotron radiation. The expression obtained illustrates the unique characteristics of multi-line TDI systems, where the finite incident energy width and use of a nonidentical emitter pair produces further information on faster sub-picosecond-scale dynamics in addition to the nanosecond dynamics; this was demonstrated experimentally. A normalized intermediate scattering function was extracted from the spectrum and its relaxation form was determined for a relaxation time of the order of 1 μs, even for relatively large momentum transfer of ~31 nm -1 . The multi-line TDI method produces a microscopic relaxation picture more rapidly and accurately than conventional single-line TDI.

  13. German neutron scattering conference. Programme and abstracts

    Energy Technology Data Exchange (ETDEWEB)

    Brueckel, Thomas (ed.)

    2012-07-01

    The German Neutron Scattering Conference 2012 - Deutsche Neutronenstreutagung DN 2012 offers a forum for the presentation and critical discussion of recent results obtained with neutron scattering and complementary techniques. The meeting is organized on behalf of the German Committee for Research with Neutrons - Komitee Forschung mit Neutronen KFN - by the Juelich Centre for Neutron Science JCNS of Forschungszentrum Juelich GmbH. In between the large European and international neutron scattering conferences ECNS (2011 in Prague) and ICNS (2013 in Edinburgh), it offers the vibrant German and international neutron community an opportunity to debate topical issues in a stimulating atmosphere. Originating from ''BMBF Verbundtreffen'' - meetings for projects funded by the German Federal Ministry of Education and Research - this conference series has a strong tradition of providing a forum for the discussion of collaborative research projects and future developments in the field of research with neutrons in general. Neutron scattering, by its very nature, is used as a powerful probe in many different disciplines and areas, from particle and condensed matter physics through to chemistry, biology, materials sciences, engineering sciences, right up to geology and cultural heritage; the German Neutron Scattering Conference thus provides a unique chance for exploring interdisciplinary research opportunities. It also serves as a showcase for recent method and instrument developments and to inform users of new advances at neutron facilities.

  14. German neutron scattering conference. Programme and abstracts

    International Nuclear Information System (INIS)

    Brueckel, Thomas

    2012-01-01

    The German Neutron Scattering Conference 2012 - Deutsche Neutronenstreutagung DN 2012 offers a forum for the presentation and critical discussion of recent results obtained with neutron scattering and complementary techniques. The meeting is organized on behalf of the German Committee for Research with Neutrons - Komitee Forschung mit Neutronen KFN - by the Juelich Centre for Neutron Science JCNS of Forschungszentrum Juelich GmbH. In between the large European and international neutron scattering conferences ECNS (2011 in Prague) and ICNS (2013 in Edinburgh), it offers the vibrant German and international neutron community an opportunity to debate topical issues in a stimulating atmosphere. Originating from ''BMBF Verbundtreffen'' - meetings for projects funded by the German Federal Ministry of Education and Research - this conference series has a strong tradition of providing a forum for the discussion of collaborative research projects and future developments in the field of research with neutrons in general. Neutron scattering, by its very nature, is used as a powerful probe in many different disciplines and areas, from particle and condensed matter physics through to chemistry, biology, materials sciences, engineering sciences, right up to geology and cultural heritage; the German Neutron Scattering Conference thus provides a unique chance for exploring interdisciplinary research opportunities. It also serves as a showcase for recent method and instrument developments and to inform users of new advances at neutron facilities.

  15. Neutron spin echo scattering angle measurement (SESAME)

    International Nuclear Information System (INIS)

    Pynn, R.; Fitzsimmons, M.R.; Fritzsche, H.; Gierlings, M.; Major, J.; Jason, A.

    2005-01-01

    We describe experiments in which the neutron spin echo technique is used to measure neutron scattering angles. We have implemented the technique, dubbed spin echo scattering angle measurement (SESAME), using thin films of Permalloy electrodeposited on silicon wafers as sources of the magnetic fields within which neutron spins precess. With 30-μm-thick films we resolve neutron scattering angles to about 0.02 deg. with neutrons of 4.66 A wavelength. This allows us to probe correlation lengths up to 200 nm in an application to small angle neutron scattering. We also demonstrate that SESAME can be used to separate specular and diffuse neutron reflection from surfaces at grazing incidence. In both of these cases, SESAME can make measurements at higher neutron intensity than is available with conventional methods because the angular resolution achieved is independent of the divergence of the neutron beam. Finally, we discuss the conditions under which SESAME might be used to probe in-plane structure in thin films and show that the method has advantages for incident neutron angles close to the critical angle because multiple scattering is automatically accounted for

  16. Neutron scattering from quantum liquids

    International Nuclear Information System (INIS)

    Cowley, R.A.

    1976-01-01

    Recent neutron scattering measurements on the quantum liquids 4 He and 3 He are described. In the Bose superfluid there is a well-defined excitation for wave vectors less than 3.6 A -1 . In the Fermi liquid measurements are much more difficult because of the large absorption cross section, but measurements at the Institute Laue-Langevin have shown that there are no well-defined excitations at 0.63 0 K for wave vectors between 1.0 and 2.6 A -1 . The difference between these results is due to the existence of particle-hole excitations in the Fermi liquid into which collective excitations can decay. Because of the simplicity of the excitations in 4 He, it has become a testing ground for the effects of the interactions between the excitations. Measurements are described which show that while roton-roton interactions are attractive at small wave vectors they are repulsive at larger wave vectors. The scattering at large momentum transfer in 4 He has been measured, but its interpretation is still open to question

  17. Electron Neutrino Charged-Current Quasielastic Scattering in the MINERvA Experiment

    Energy Technology Data Exchange (ETDEWEB)

    Wolcott, Jeremy [Rochester U.

    2015-10-28

    The electron-neutrino charged-current quasielastic (CCQE) cross section on nuclei is an important input parameter to appearance-type neutrino oscillation experiments. Current experiments typically work from the muon neutrino cross section and apply corrections from theoretical arguments to obtain a prediction for the electron neutrino cross section, but to date there has been no experimental verification of the estimates for this channel at an energy scale appropriate to such experiments. We present the first measurement of an exclusive reaction in few-GeV electron neutrino interactions, namely, the cross section for a CCQE-like process, made using the MINERvA detector. The result is given as differential cross-sections vs. the electron energy, electron angle, and square of the four-momentum transferred to the nucleus, $Q^2$. We also compute the ratio to a muon neutrino cross-section in $Q^2$ from MINERvA. We find satisfactory agreement between this measurement and the predictions of the GENIE generator.

  18. La nouvelle vague in polarized neutron scattering

    International Nuclear Information System (INIS)

    Mezei, F.

    1986-01-01

    Polarized neutron research, like many other subjects in neutron scattering developed in the footsteps of Cliff Shull. The classical polarized neutron technique he pioneered was generalized around 1970 to vectorial beam polarizations and this opened up the way to a ''nouvelle vague'' of neutron scattering experiments. In this paper I will first reexamine the old controversy on the question whether the nature of the neutron magnetic moment is that of a microscopic dipole or of an Amperian current loop. The problem is not only of historical interest, but also of relevance to modern applications. This will be followed by a review of the fundamentals on spin coherence effects in neutron beams and scattering, which are the basis of vectorial beam polarization work. As an example of practical importance, paramagnetic scattering will be discussed. The paper concludes with some examples of applications of the vector polarization techniques, such as study of ferromagnetic domains by neutron beam depolarization and Neutron Spin Echo high resolution inelastic spectroscopy. The sample results presented demonstrate the new opportunities this novel approach opened up in neutrons scattering research. (orig.)

  19. Neutron scattering in Indonesia. Country report

    Energy Technology Data Exchange (ETDEWEB)

    Ikram, Abarrul [Neutron Scattering Laboratory, R and D Center for Materials Science and Technology, National Nuclear Energy Agency, Serpong (Indonesia)

    2000-10-01

    Neutron scattering in Indonesia is still alienated due to some reasons and conditions which are discussed. The reactor and its latest operation mode are also described. The neutron beam facilities which include one diffractometer for residual stress measurement, one diffractometer for single crystal structural determination and texture measurement, one high resolution powder diffractometer, one neutron radiography facility, one triple axis spectrometer, one small angle neutron scattering spectrometer and one high resolution small angle neutron scattering spectrometer were presented briefly together with improvements of neutron intensities at some spectrometers in connection with the setting of main beam shutter position. Special attention is given for four instruments mostly related to this workshop. Their performances and problems faced in the past 9 months are presented as well as the future plan for refurbishment and development. (author)

  20. Neutrons scattering studies in the actinide region

    International Nuclear Information System (INIS)

    Kegel, G.H.R.; Egan, J.J.

    1992-09-01

    During the report period were investigated the following areas: prompt fission neutron energy spectra measurements; neutron elastic and inelastic scattering from 239 Pu; neutron scattering in 181 Ta and 197 Au; response of a 235 U fission chamber near reaction thresholds; two-parameter data acquisition system; ''black'' neutron detector; investigation of neutron-induced defects in silicon dioxide; and multiple scattering corrections. Four Ph.D. dissertations and one M.S. thesis were completed during the report period. Publications consisted of three journal articles, four conference papers in proceedings, and eleven abstracts of presentations at scientific meetings. There are currently four Ph.D. and one M.S. candidates working on dissertations directly associated with the project. In addition, three other Ph.D. candidates are working on dissertations involving other aspects of neutron physics in this laboratory

  1. Scattering of fast neutrons from elemental molybdenum

    International Nuclear Information System (INIS)

    Smith, A.B.; Guenther, P.T.

    1982-11-01

    Differential broad-resolution neutron-scattering cross sections of elemental molybdenum were measured at 10 to 20 scattering angles distributed between 20 and 160 degrees and at incident-neutron energy intervals of approx. = 50 to 200 keV from 1.5 to 4.0 MeV. Elastically-scattered neutrons were fully resolved from inelastic events. Lumped-level inelastic-neutron-scattering cross sections were determined corresponding to observed excitation energies of; 789 +- 23, 195 +- 23, 1500 +- 34, 1617 +- 12, 1787, 1874, 1991, 2063 +- 24, 2296, 2569 and 2802 keV. An optical-statistical model was deduced from the measured elastic-scattering results. The experimental values were compared with the respective quantities given in ENDF/B-V

  2. Dynamics and denaturation of a protein. Simulations and neutron scattering on staphylococcus nuclease

    International Nuclear Information System (INIS)

    Goupil-Lamy, Anne

    1997-01-01

    This research thesis reports simulations and experiments of inelastic scattering on the whole frequency spectrum to analyse the vibrations of the staphylococcus nuclease and its fragment, in order to study protein folding. Based on these experiments, information on eigenvectors which describe vibration modes can be directly obtained. Inelastic intensities are indeed fully determined by nuclear cross sections and the mean square displacement of each atom. Some experimentally noticed peaks are then explained by calculating a theoretical spectrum from an analysis of normal modes. The studied fragment is made of 136 c-terminal residues. The fragment structure obtained by molecular dynamics simulation is compared with available experimental data. Then, experiments of neutron scattering on the nuclease of staphylococcus and its fragment have been performed. Quasi elastic scattering spectra have been measured. The author then used simulations to try to reproduce the quasi-elastic spectrum. Experiments of inelastic scattering have then been performed [fr

  3. Very High Energy Neutron Scattering from Hydrogen

    International Nuclear Information System (INIS)

    Cowley, R A; Stock, C; Bennington, S M; Taylor, J; Gidopoulos, N I

    2010-01-01

    The neutron scattering from hydrogen in polythene has been measured with the direct time-of flight spectrometer, MARI, at the ISIS facility of the Rutherford Appleton Laboratory with incident neutron energies between 0.5 eV and 600 eV. The results of experiments using the spectrometer, VESUVIO, have given intensities from hydrogen containing materials that were about 60% of the intensity expected from hydrogen. Since VESUVIO is the only instrument in the world that routinely operates with incident neutron energies in the eV range we have chosen to measure the scattering from hydrogen at high incident neutron energies with a different type of instrument. The MARI, direct time-of-flight, instrument was chosen for the experiment and we have studied the scattering for several different incident neutron energies. We have learnt how to subtract the gamma ray background, how to calibrate the incident energy and how to convert the spectra to an energy plot . The intensity of the hydrogen scattering was independent of the scattering angle for scattering angles from about 5 degrees up to 70 degrees for at least 3 different incident neutron energies between 20 eV and 100 eV. When the data was put on an absolute scale, by measuring the scattering from 5 metal foils with known thicknesses under the same conditions we found that the absolute intensity of the scattering from the hydrogen was in agreement with that expected to an accuracy of ± 5.0% over a wide range of wave-vector transfers between 1 and 250 A -1 . These measurements show that it is possible to measure the neutron scattering with incident neutron energies up to at least 100 eV with a direct geometry time-of-flight spectrometer and that the results are in agreement with conventional scattering theory.

  4. Neutron scattering studies of solid electrolytes

    International Nuclear Information System (INIS)

    Shapiro, S.M.

    1976-01-01

    The role which neutron scattering can play in determining the nature of the disorder and the conducting mechanism in the solid electrolytes is discussed. First, some of the general formalism for elastic and inelastic neutron scattering is reviewed, and the quantities which can be measured are pointed out. Then the application of neutron scattering to the studies of three different problems is examined; the anion disorder in the fluorite system, the dynamical behavior in beta-alumina, and the cation diffusion in αAgI are discussed. 8 figures

  5. Techniques in high pressure neutron scattering

    CERN Document Server

    Klotz, Stefan

    2013-01-01

    Drawing on the author's practical work from the last 20 years, Techniques in High Pressure Neutron Scattering is one of the first books to gather recent methods that allow neutron scattering well beyond 10 GPa. The author shows how neutron scattering has to be adapted to the pressure range and type of measurement.Suitable for both newcomers and experienced high pressure scientists and engineers, the book describes various solutions spanning two to three orders of magnitude in pressure that have emerged in the past three decades. Many engineering concepts are illustrated through examples of rea

  6. Monte Carlo simulations of neutron scattering instruments

    International Nuclear Information System (INIS)

    Aestrand, Per-Olof; Copenhagen Univ.; Lefmann, K.; Nielsen, K.

    2001-01-01

    A Monte Carlo simulation is an important computational tool used in many areas of science and engineering. The use of Monte Carlo techniques for simulating neutron scattering instruments is discussed. The basic ideas, techniques and approximations are presented. Since the construction of a neutron scattering instrument is very expensive, Monte Carlo software used for design of instruments have to be validated and tested extensively. The McStas software was designed with these aspects in mind and some of the basic principles of the McStas software will be discussed. Finally, some future prospects are discussed for using Monte Carlo simulations in optimizing neutron scattering experiments. (R.P.)

  7. Using quasi-elastic neutron diffraction to study positive electrode for lithium and sodium-ion batteries

    International Nuclear Information System (INIS)

    Pramudita, James C.; Sharma, Neeraj

    2015-01-01

    Sodium-ion batteries has recently been proposed as the alternative for lithium-ion batteries to be the low cost energy storage system. However, challenges still remains for the development of sodium-ion batteries. Optimization of electrode materials and electrolyte capable of insertion/extraction of sodium-ion in a safe and economic way under high current density is needed in order to produce commercially viable sodium-ion batteries. While possible positive electrode material is more prevalent than negative electrode material, many of these material still need further understanding. Quasi-elastic Neutron Scatteringis a technique that utilize the inelastic Neutron Scatteringthat can be used to study solid-state diffusion in materials. This technique can be used to study the diffusion of sodium-ion under electric field through the electrolyte and positive electrode materials in order to further understand the mechanism of sodium insertion/extraction in a working battery. This technique can also be used to study available positive electrode material for lithium-ion batteries to further understand the mechanism of lithium-ion diffusion in current working lithiumion batteries.

  8. Current status of neutron scattering in Thailand

    International Nuclear Information System (INIS)

    Kornduangkaeo, Areeratt; Pongkasem, Somchai; Putchar, Suriya; Ampornrat, Pantip; Kajornrith, Varavuth; Chamchang, Jipawat

    2006-01-01

    The current neutron powder diffractometer at the Thai Research Reactor-1/Modification 1 (TRR-1/M1) has been modified from the obsolete neutron diffractometer which had been used during 1968-1975. The upgraded diffractometer has medium resolution and is appropriate for studying samples with small unit cell dimensions and training university students in the field of neutron scattering. This paper describes the current activities of neutron scattering research in Thailand, the current status of a new research reactor project at Ongkarak for enlarging the perspectives of its utilization in the future as well as the organizational reformation of the Office of Atomic Energy for Peace (OAEP). (author)

  9. Current status of neutron scattering in Thailand

    International Nuclear Information System (INIS)

    Kornduangkaeo, Areeratt; Pongkasem, Somchai; Putchar, Suriya; Ampornrat, Pantip; Kajornrith, Varavuth; Sangariyavanich, Archara

    2003-01-01

    The current neutron powder diffractometer at the Thai Research Reactor-1/M1 (TRR-1/M1) has been modified from the obsolete neutron diffractometer which had been used during 1968-1975. The upgraded diffractometer has medium resolution and is appropriate for studying samples with small unit cell dimensions and training university students in the field of neutron scattering. This paper describes the current activities of neutron scattering research in Thailand as well as a new research reactor for enlarging the perspectives of its utilization in the future. (author)

  10. Neutron-scattering studies of the S=2 antiferromagnetic chain MnCl3(C10D8N2)

    International Nuclear Information System (INIS)

    Granroth, G.E.; Nagler, S.E.; Coldea, R.; Eccleston, R.S.; Ward, B.H.; Talham, D.R.; Meisel, M.W.

    2002-01-01

    Quasi-elastic and inelastic neutron scattering studies of the quasi-one-dimensional S=2 antiferromagnet MnCl 3 (C 10 D 8 N 2 ) are reported. The quasi-elastic measurements exhibit a broad peak at Q∼0.69 A -1 , which is consistent with short-range antiferromagnetic coupling between neighboring Mn 3+ ions. Inelastic experiments, at 150 mK and Q=0.70 A -1 , reveal decreased magnetic scattering at energies less than 0.2 meV when compared to similar studies at 20 K. These results provide microscopic evidence for the presence of a Haldane gap and are consistent with the bulk magnetization measurements of Granroth et al. (orig.)

  11. Measurement of the Antineutrino Double-Differential Charged-Current Quasi-Elastic Scattering Cross Section at MINERvA

    Energy Technology Data Exchange (ETDEWEB)

    Patrick, Cheryl [Northwestern U.

    2016-01-01

    Next-generation neutrino oscillation experiments, such as DUNE and Hyper-Kamiokande, hope to measure charge-parity (CP) violation in the lepton sector. In order to do this, they must dramatically reduce their current levels of uncertainty, particularly those due to neutrino-nucleus interaction models. As CP violation is a measure of the difference between the oscillation properties of neutrinos and antineutrinos, data about how the less-studied antineutrinos interact is especially valuable. We present the MINERvA experiment's first double-differential scattering cross sections for antineutrinos on scintillator, in the few-GeV range relevant to experiments such as DUNE and NOvA. We also present total antineutrino-scintillator quasi-elastic cross sections as a function of energy, which we compare to measurements from previous experiments. As well as being useful to help reduce oscillation experiments' uncertainty, our data can also be used to study the prevalence of various cor relation and final-state interaction effects within the nucleus. We compare to models produced by different model generators, and are able to draw first conclusions about the predictions of these models.

  12. Effects of Pressure on Stability of Biomolecules in Solutions Studied by Neutron Scattering

    Science.gov (United States)

    Bellissent-Funel, Marie-Claire-; Appavou, Marie-Sousai; Gibrat, Gabriel

    Studies of the pressure dependence on protein structure and dynamics contribute not only to the basic knowledge of biological molecules but have also a considerable relevance in full technology, like in food sterilization and pharmacy. Conformational changes induced by pressure as well as the effects on the protein stability have been mostly studied by optical techniques (optical absorption, fluorescence, phosphorescence), and by NMR. Most optical techniques used so far give information related to the local nature of the used probe (fluorescent or phosphorescent tryptophan). Small angle neutron scattering and quasi-elastic neutron scattering provide essential complementary information to the optical data, giving quantitative data on change of conformation of soluble globular proteins such as bovine pancreatic trypsin inhibitor (BPTI) and on the mobility of protons belonging to the protein surface residues.

  13. Aspects of molecular dynamic of cyclohexanol studied by scattering of slow neutrons

    International Nuclear Information System (INIS)

    Walder, Vilma Sidneia

    1978-01-01

    Molecular dynamics of cyclohexanol in three crystalline phases and in the liquid state was investigated by cold neutron scattering in the temperature interval 100 to 300 K. The measurements were performed using a Beryllium Filter Time-of-Flight Spectrometer. The neutron inelastic scattering spectra and the frequency spectra fitted by a sum of Gaussians show evidences for events around 36-44. 62-79, 120-148, 216-250 and 384-509 c m -1 interpreted respectively as hundred rotation of molecules, lattice vibrations, H bond stretching vibration, out-of-line and in-plane ring bending modes. Quasi-elastic broadening were analysed in terms of modules for molecular diffusion. The behaviour of the self-diffusion coefficient with temperature was studied and the activation energies for diffusion in the liquid and solid states were determined. (author)

  14. Advantages of neutron scattering for biological structure analysis

    International Nuclear Information System (INIS)

    Schoenborn, B.P.

    1975-01-01

    The advantages and disadvantages of neutron scattering for protein crystallography, scattering from oriented systems, and solution scattering are summarized. Techniques for minimizing the disadvantages are indicated

  15. Anomalous neutron scattering and feroelectric modes

    International Nuclear Information System (INIS)

    Viswanathan, K.S.

    1977-01-01

    It is suggested that anomalous neutron scattering could prove a powerful experimental tool in studying ferroelectric phase transition, the sublattice displacements of the soft modes as well as their symmetry characteristics. (author)

  16. Neutron scattering for studies of soft matter at SNS and HFIR

    International Nuclear Information System (INIS)

    Smith, Gregory S.

    2013-01-01

    In this talk, we will present an overview of the scientific program of the Structure and Dynamics of Soft Matter Group, in the Biology and Soft Matter Division of the Neutron Sciences Directorate. From the broader area of soft materials research, the group members have chosen four main areas of scientific focus including: Confinement and Low-Dimensional Systems, Structure and Dynamics of Colloids, Nanoparticle-Polymer Composites, Transport in Membranes, and New Neutron Techniques for soft matter science. We will present several examples of neutron scattering experimental studies in each of these areas highlighting the experimental and theoretical (or modeling) capabilities of the group at both HFIR and SNS. Example topics to be discussed include SANS, reflectometry, and/or quasielastic studies of membranes on patterned interfaces, dynamics and structure of soft colloidal materials (including both polymeric dendrimers and biomimetic materials), gas confinement in mesoporous structures, transport in polyelectrolyte thin films, and development of spin-echo SANS concepts. (author)

  17. Neutron Scattering studies of magnetic molecular magnets

    International Nuclear Information System (INIS)

    Chaboussant, G.

    2009-01-01

    This work deals with inelastic neutron scattering studies of magnetic molecular magnets and focuses on their magnetic properties at low temperature and low energies. Several molecular magnets (Mn 12 , V 15 , Ni 12 , Mn 4 , etc.) are reviewed. Inelastic neutron scattering is shown to be a perfectly suited spectroscopy tool to -a) probe magnetic energy levels in such systems and -b) provide key information to understand the quantum tunnel effect of the magnetization in molecular spin clusters. (author)

  18. Progress report on neutron scattering at JAERI

    Energy Technology Data Exchange (ETDEWEB)

    Morii, Yukio [Japan Atomic Energy Research Inst., Tokai, Ibaraki (Japan). Tokai Research Establishment

    1998-10-01

    In the first half of fiscal year 1997, JRR-3M was operated for 97 days followed by a long term shut down for its annual maintenance. Three days were lost out of 100 scheduled operation days, due to a trouble in irradiation facility. Neutron scattering research activities at the JRR-3M have been extended from that of fiscal year 1996. In the Research Group for Quantum Condensed Matter System, experimental study under high pressures, low temperatures and high fields as well as coupling of these conditions were planned to find new quantum condensed matter systems. And, obtained experimental results were immediately provided to theorists for their investigations. In cooperation with new group, Research Group for Neutron Scattering of Strongly Correlated Electron Systems and Research Group for Neutron Scattering at Ultralow Temperatures were carrying neutron scattering experiments at JRR-3M. Research Group for Neutron Crystallography in Biology had opened a way for investigating biomatter neutron diffraction research with high experimental accuracy by growing a millimeter-class large single crystal. In fiscal year 1997, 39 research projects were conducted by these four groups and other staffs in JAERI, 27 projects collaborated with university researchers and 3 projects collaborated with private enterprises were also conducted as complementary researches. 2117 days of machine times were requested to use 8 neutron scattering instruments this year, which corresponded to 1.51 times larger than those planned at its beginning. (G.K.)

  19. Scattering of Neutrons by an Anharmonic Crystal

    Energy Technology Data Exchange (ETDEWEB)

    Hoegberg, T; Bohlin, L; Ebbsjoe, I

    1967-04-15

    Numerical calculations have been performed for the anharmonic effects in neutron scattering. The phonon frequency widths and shifts have been calculated as a function of neutron frequency at different wave numbers and temperatures for a potential with central symmetry and for a face-centered cubic lattice.

  20. Status and neutron scattering experiments at KENS

    International Nuclear Information System (INIS)

    Watanabe, N.; Sasaki, H.; Ishikawa, Y.; Endoh, Y.; Inoue, K.

    1983-01-01

    This paper reports present status of the KENS facility, progress in neutron scattering experiments and instrumental developments, and status of the KENS-I' program. A design study of a high intensity rapid-cycle 800 MeV proton synchrotron for proposed new pulsed neutron (KENS-II) and meson source is also descirbed

  1. Lectures on magnetism and neutron scattering

    International Nuclear Information System (INIS)

    Gunn, J.M.F.

    1983-12-01

    The paper contains six lectures given to the Neutron Division of the Rutherford Appleton laboratory in 1983. The aim was to explain fundamental physics of neutron scattering and basic magnetism to the non-specialist scientist. The text includes: origin of neutron's magnetic moment and spin-dependent interactions with electrons and nuclei, why are solids magnetic, magnetic anistropy and domain structure, phenomenological spin waves, magnetic phase transitions and electronic excitations in magnets. (U.K.)

  2. Ramsauer effect in triplet neutron-neutron scattering

    International Nuclear Information System (INIS)

    Pupyshev, V.V.; Solovtsova, O.P.

    1995-01-01

    As we show, due to interplay of pure nuclear and magnetic moment interactions, the total cross section of triplet neutron-neutron scattering should possess a non-zero limit at E cm = 0 and a local minimum at ∼ 20 keV. 17 refs., 1 fig

  3. Introduction to neutron scattering. Lecture notes of the introductory course

    International Nuclear Information System (INIS)

    Furrer, A.

    1996-01-01

    These proceedings enclose ten papers presented at the 1. European Conference on Neutron scattering (ECNS '96). The aim of the Introductory Course was fourfold: - to learn the basic principles of neutron scattering, - to get introduced into the most important classes of neutron scattering instruments, -to learn concepts and their transformation into neutron scattering experiments in various fields of condensed matter research, - to recognize the limitations of the neutron scattering technique as well as to the complementarity of other methods. figs., tabs., refs

  4. Neutron scattering by normal liquids

    Energy Technology Data Exchange (ETDEWEB)

    Gennes, P.G. de [Commissariat a l' Energie Atomique, Saclay (France). Centre d' Etudes Nucleaires

    1961-07-01

    Neutron data on motions in normal liquids well below critical point are reviewed and classified according to the order of magnitude of momentum transfers {Dirac_h}q and energy transfers {Dirac_h}w. For large momentum transfers a perfect gas model is valid. For smaller q and incoherent scattering, the major effects are related to the existence of two characteristic times: the period of oscillation of an atom in its cell, and the average lifetime of the atom in a definite cell. Various interpolation schemes covering both time scales are discussed. For coherent scattering and intermediate q, the energy spread is expected to show a minimum whenever q corresponds to a diffraction peak. For very small q the standard macroscopic description of density fluctuations is applicable. The limits of the various (q) and (w) domains and the validity of various approximations are discussed by a method of moments. The possibility of observing discrete transitions due to internal degrees of freedom in polyatomic molecules, in spite of the 'Doppler width' caused by translational motions, is also examined. (author) [French] L'auteur examine les donnees neutroniques sur les mouvements dans les liquides normaux, bien au-dessous du point critique, et les classe d'apres l'ordre de grandeur des transferts de quantite de mouvement {Dirac_h}q et des transferts d'energie {Dirac_h}w. Pour les grands transferts de, quantite de mouvement, un modele de gaz parfait est valable. En ce qui concerne les faibles valeurs de q et la diffussion incoherente, les principaux effets sont lies a l'existence de deux temps caracteristiques: la periode d'oscillation d'un atome dans sa cellule et la duree moyenne de vie de l'atome dans une cellule determinee. L'auteur etudie divers systemes d'interpolation se rapportant aux deux echelles de temps. Pour la diffusion coherente et les valeurs intermediaires de q, on presume que le spectre d'energie accuse un minimum chaque fois que q correspond a un pic de

  5. Neutron Scattering from 36Ar and 4He Films

    DEFF Research Database (Denmark)

    Carneiro, K.

    1977-01-01

    Scale factors for neutron diffraction and neutron inelastic scattering are presented for common adsorbates, and the feasibility of experiments is discussed together with the information gained by each type of experiment. Diffraction, coherent inelastic scattering, and incoherent scattering are tr...

  6. Sub-barrier fusion and near-barrier quasi-elastic scattering

    International Nuclear Information System (INIS)

    Kolata, J.J.; Tighe, R.J.

    1990-01-01

    Elastic scattering of 32 S on 58,64 Ni and fusion of 32 S+ 58,64 Ni and 34 S+ 64 Ni have been measured at energies near the Coulomb barrier. Our results differ in several important respects from previous measurements on these systems. Coupled-channels calculations which explicitly allow for inelastic excitation and single-nucleon transfer reproduce the main features of the new data. Near-barrier elastic scattering of 48 Ca on 40 Ca has also been measured. These data provide evidence for the effect of strong coupling to positive Q-value channels other than single-nucleon transfer. 18 refs., 3 figs

  7. Neutron Scattering in Biology Techniques and Applications

    CERN Document Server

    Fitter, Jörg; Katsaras, John

    2006-01-01

    The advent of new neutron facilities and the improvement of existing sources and instruments world wide supply the biological community with many new opportunities in the areas of structural biology and biological physics. The present volume offers a clear description of the various neutron-scattering techniques currently being used to answer biologically relevant questions. Their utility is illustrated through examples by some of the leading researchers in the field of neutron scattering. This volume will be a reference for researchers and a step-by-step guide for young scientists entering the field and the advanced graduate student.

  8. Diffuse neutron scattering signatures of rough films

    International Nuclear Information System (INIS)

    Pynn, R.; Lujan, M. Jr.

    1992-01-01

    Patterns of diffuse neutron scattering from thin films are calculated from a perturbation expansion based on the distorted-wave Born approximation. Diffuse fringes can be categorised into three types: those that occur at constant values of the incident or scattered neutron wavevectors, and those for which the neutron wavevector transfer perpendicular to the film is constant. The variation of intensity along these fringes can be used to deduce the spectrum of surface roughness for the film and the degree of correlation between the film's rough surfaces

  9. Fast-neutron scattering from elemental cadmium

    International Nuclear Information System (INIS)

    Smith, A.B.; Guenther, P.T.

    1982-07-01

    Neutron differential-elastic-scattering cross sections of elemental cadmium are measured from approx. = 1.5 to 4.0 MeV at incident-neutron energy intervals of 50 to 200 keV and at 10 to 20 scattering angles distributed between approx. = 20 and 160 degrees. Concurrently, lumped-level neutron inelastic-excitation cross sections are measured. The experimental results are used to deduce parameters of an optical-statistical model that is descriptive of the observables and are compared with corresponding quantities given in ENDF/B-V

  10. Neutron scattering instruments for the Spallation Neutron Source (SNS)

    International Nuclear Information System (INIS)

    Crawford, R.K.; Fornek, T.; Herwig, K.W.

    1998-01-01

    The Spallation Neutron Source (SNS) is a 1 MW pulsed spallation source for neutron scattering planned for construction at Oak Ridge National Laboratory. This facility is being designed as a 5-laboratory collaboration project. This paper addresses the proposed facility layout, the process for selection and construction of neutron scattering instruments at the SNS, the initial planning done on the basis of a reference set of ten instruments, and the plans for research and development (R and D) to support construction of the first ten instruments and to establish the infrastructure to support later development and construction of additional instruments

  11. Effects of hadronic colour structure in quasi-elastic and charge-exchange scattering on nuclei

    International Nuclear Information System (INIS)

    Kopeliovich, B.Z.; Zakharov, B.G.

    1986-01-01

    Effects of hadronic hidden colour screening are considered in hadron-nucleus interaction. It is shown that in the quasi-free charge exchange-reaction nuclear matter becomes transparent for the scattered hadron if the momentum transfer is large enough. The available experimental data confirm this prediction of QCD

  12. Small angle neutron scattering by polymer solutions

    International Nuclear Information System (INIS)

    Farnoux, B.; Jannink, G.

    1980-08-01

    Small angle neutron scattering is an experimental technique introduced since about 10 years for the observation of the polymer conformation in all the concentration range from dilute solution to the melt. After a brief recall of the elementary relations between scattering amplitude, index of refraction and scattered intensity, two concepts related to this last quantity (the contrast and the pair correlation function) are discussed in details

  13. Inelastic neutron scattering from cerium under pressure

    International Nuclear Information System (INIS)

    Rainford, B.D.; Buras, B.; Lebech, B.

    1976-01-01

    Inelastic neutron scattering from Ce metal at 300K was studied both below and above the first order γ-α phase transition, using a triple axis spectrometer. It was found that (a) there is no indication of any residual magnetic scattering in the collapsed α phase and (b) the energy width of the paramagnetic scattering in the γ-phase increases with pressure. (Auth.)

  14. Zeeman splitting of surface-scattered neutrons

    International Nuclear Information System (INIS)

    Felcher, G.P.; Adenwalla, S.; De Haan, V.O.; Van Well, A.A.

    1995-01-01

    If a beam of slow neutrons impinges on a solid at grazing incidence, the neutrons reflected can be used to probe the composition and magnetization of the solid near its surface. In this process, the incident and reflected neutrons generally have identical kinetic energies. Here we report the results of an experiment in which subtle inelastic scattering processes are revealed as relatively large deviations in scattering angle. The neutrons are scattered from a ferromagnetic surface in the presence of a strong ambient magnetic field, and exhibit a small but significant variation in kinetic energy as a function of the reflection angle. This effect is attributable to the Zeeman splitting of the energies of the neutron spin states due to the ambient magnetic field: some neutrons flip their spins upon reflection from the magnetized surface, thereby exchanging kinetic energy for magnetic potential energy. The subtle effects of Zeeman splitting are amplified by the extreme sensitivity of grazing-angle neutron scattering, and might also provide a useful spectroscopic tool if significant practical obstacles (such as low interaction cross-sections) can be overcome. (author)

  15. Neutron Brillouin scattering in dense fluids

    Energy Technology Data Exchange (ETDEWEB)

    Verkerk, P [Technische Univ. Delft (Netherlands); FINGO Collaboration

    1997-04-01

    Thermal neutron scattering is a typical microscopic probe for investigating dynamics and structure in condensed matter. In contrast, light (Brillouin) scattering with its three orders of magnitude larger wavelength is a typical macroscopic probe. In a series of experiments using the improved small-angle facility of IN5 a significant step forward is made towards reducing the gap between the two. For the first time the transition from the conventional single line in the neutron spectrum scattered by a fluid to the Rayleigh-Brillouin triplet known from light-scattering experiments is clearly and unambiguously observed in the raw neutron data without applying any corrections. Results of these experiments are presented. (author).

  16. Polarized neutron scattering research: the beginning

    International Nuclear Information System (INIS)

    Mezei, F.

    2005-01-01

    The visionary idea of using neutron scattering for the study of magnetic phenomena in condensed matter was proposed by Bloch in 1936, mere 4 years after the neutron was discovered. It was based on one of the surprises the neutron presented the scientific community with: it is neutral, yet it has a magnetic moment, which latter was then not yet directly observed though. Although the first results proved to be mathematically wrong, due to a non-trivial ambiguity of classical electromagnetism theory, which could only be settled by neutron beam experiments 15 years later, the recognition lead to the advent of a most productive area of modern research, which culminated in the development of the powerful and sophisticated techniques of polarized neutron scattering. This recollection traces the early milestones of the development of the field in strong interaction between theory and experiment

  17. Heavy ion elastic and quasi-elastic scattering above E/A = 30 MeV

    International Nuclear Information System (INIS)

    Barrette, J.

    1986-05-01

    At high energy, heavy-ion elastic scattering probes the ion-ion potential in a large domain much inside the strong absorption radius. This results in a more precise determination of the real part of the nuclear potential and a consistent picture of its evolution with energy begins to emerge. It is relatively similar to that observed in light ion scattering. Even if the inelastic angular distributions seem to contain less refractive or interior contribution, coupled channel effects from these states are still important at least up to 20 MeV/n. Heavy-ion induced transfer reactions to discrete states have small cross sections but present a very strong selectivity for states with the highest available spin and could thus provide new and interesting spectroscopic information

  18. BUILDING A NETWORK FOR NEUTRON SCATTERING EDUCATION

    International Nuclear Information System (INIS)

    Pynn, Roger; Baker, Shenda Mary; Louca, Despo A.; McGreevy, Robert L.; Ekkebus, Allen E.; Kszos, Lynn A.; Anderson, Ian S.

    2008-01-01

    In a concerted effort supported by the National Science Foundation, the Department of Commerce, and the Department of Energy, the United States is rebuilding its leadership in neutron scattering capability through a significant investment in U.S. neutron scattering user facilities and related instrumentation. These unique facilities provide opportunities in neutron scattering to a broad community of researchers from academic institutions, federal laboratories, and industry. However, neutron scattering is often considered to be a tool for 'experts only' and in order for the U.S. research community to take full advantage of these new and powerful tools, a comprehensive education and outreach program must be developed. The workshop described below is the first step in developing a national program that takes full advantage of modern education methods and leverages the existing educational capacity at universities and national facilities. During March 27-28, 2008, a workshop entitled 'Building a Network for Neutron Scattering Education' was held in Washington, D.C. The goal of the workshop was to define and design a roadmap for a comprehensive neutron scattering education program in the United States. Successful implementation of the roadmap will maximize the national intellectual capital in neutron sciences and will increase the sophistication of research questions addressed by neutron scattering at the nation's forefront facilities. (See Appendix A for the list of attendees, Appendix B for the workshop agenda, Appendix C for a list of references. Appendix D contains the results of a survey given at the workshop; Appendix E contains summaries of the contributed talks.) The workshop brought together U.S. academicians, representatives from neutron sources, scientists who have developed nontraditional educational programs, educational specialists, and managers from government agencies to create a national structure for providing ongoing neutron scattering education. A

  19. BUILDING A NETWORK FOR NEUTRON SCATTERING EDUCATION

    Energy Technology Data Exchange (ETDEWEB)

    Pynn, Roger [ORNL; Baker, Shenda Mary [ORNL; Louca, Despo A [ORNL; McGreevy, Robert L [ORNL; Ekkebus, Allen E [ORNL; Kszos, Lynn A [ORNL; Anderson, Ian S [ORNL

    2008-10-01

    In a concerted effort supported by the National Science Foundation, the Department of Commerce, and the Department of Energy, the United States is rebuilding its leadership in neutron scattering capability through a significant investment in U.S. neutron scattering user facilities and related instrumentation. These unique facilities provide opportunities in neutron scattering to a broad community of researchers from academic institutions, federal laboratories, and industry. However, neutron scattering is often considered to be a tool for 'experts only' and in order for the U.S. research community to take full advantage of these new and powerful tools, a comprehensive education and outreach program must be developed. The workshop described below is the first step in developing a national program that takes full advantage of modern education methods and leverages the existing educational capacity at universities and national facilities. During March 27-28, 2008, a workshop entitled 'Building a Network for Neutron Scattering Education' was held in Washington, D.C. The goal of the workshop was to define and design a roadmap for a comprehensive neutron scattering education program in the United States. Successful implementation of the roadmap will maximize the national intellectual capital in neutron sciences and will increase the sophistication of research questions addressed by neutron scattering at the nation's forefront facilities. (See Appendix A for the list of attendees, Appendix B for the workshop agenda, Appendix C for a list of references. Appendix D contains the results of a survey given at the workshop; Appendix E contains summaries of the contributed talks.) The workshop brought together U.S. academicians, representatives from neutron sources, scientists who have developed nontraditional educational programs, educational specialists, and managers from government agencies to create a national structure for providing ongoing neutron

  20. Phenylene ring dynamics in bisphenol-A-polysulfone by neutron scattering

    International Nuclear Information System (INIS)

    Arrese-Igor, S.; Arbe, A.; Alegria, A.; Colmenero, J.; Frick, B.

    2004-01-01

    We have investigated the dynamics of phenylene rings in a glassy polysulfone (bisphenol-A-polysulfone) by means of quasielastic neutron scattering. Nowadays it is well known that these molecular motions are directly connected with the mechanical properties of engineering thermoplastics in general. The particular system investigated by us has the advantage that by selective deuteration of the methyl groups, the neutron scattering measured is dominated by the incoherent contribution from the protons in the phenylene rings. In this way, the dynamics of such molecular groups can be experimentally isolated. Two different types of neutron spectrometers: time of flight and backscattering, were used in order to cover a wide dynamic range, which extends from microscopic (10 -13 s) to mesoscopic (10 -9 s) times. Moreover, neutron diffraction experiments with polarization analysis were also carried out in order to characterize the structural features of the sample investigated. Fast oscillations of increasing amplitude with temperature and π-flips are identified for phenylene rings motions. Due to the structural disorder characteristic of the amorphous state, both molecular motions display a broad distribution of relaxation times, which spreads over several orders of magnitude. Based on the results obtained, we propose a model for phenylene rings dynamics, which combines the two kinds of molecular motions identified. This model nicely describes the neutron scattering results in the whole dynamic range investigated

  1. Current status of neutron scattering in Thailand

    International Nuclear Information System (INIS)

    Ampornrat, Pantip

    2000-01-01

    The neutron scattering experiments in Thailand have been done continuously since the start up of the reactor. In 1977, Thai research reactor was modified into TRIGA MARK III core. After that, the neutron spectrometer was installed again under a development program. Installation of upgrading spectrometer was delayed because of some problems involving the neutron intensity and instruments. However, these problems were solved and the setup is almost completed. The paper reports the current status of neutron spectrometer, the problems and plans for the experiments. (author)

  2. Study of the atomic motion in methanol by slow neutron scattering

    International Nuclear Information System (INIS)

    Rodrigues, C.

    1979-01-01

    Cold neutron scattering data are reported for methyl alcohol in the liquid phase at room temperature. The quasielastic scattering was interpreted using the Larsson and Bergstedt model, that takes into account intramolecular motions and molecular diffusion. On the basis of this model, one finds for the relaxation time of the hindered rotation of the CH 3 group within the molecule a value 2,4 x 10 -12 sec. The analysis of the quasielastic scattering to the L-B model explain in a consistent way our experimental results in a range of momentum transfers of about 0.80 - 1.55A -1 . In the inelastic region some structure is observed at energy transfers of 22, 17 and 5 meV. The 17 meV energy transfer is associated with the 1→0 transition of the torsional oscillations of the methyl group. The activation energy for the above motion was calculated to be E=1.3 kcal/mol, in good agreement with the value of the barrier height for internal rotation of the CH 3 in methanol, obtained by microwave methods. (Author) [pt

  3. Neutron scattering studies of modulated magnetic structures

    Energy Technology Data Exchange (ETDEWEB)

    Aagaard Soerensen, Steen

    1999-08-01

    This report describes investigations of the magnetic systems DyFe{sub 4}Al{sub 8} and MnSi by neutron scattering and in the former case also by X-ray magnetic resonant scattering. The report is divided into three parts: An introduction to the technique of neutron scattering with special emphasis on the relation between the scattering cross section and the correlations between the scattering entities of the sample. The theoretical framework of neutron scattering experiments using polarized beam technique is outlined. The second part describes neutron and X-ray scattering investigation of the magnetic structures of DyFe{sub 4}Al{sub 8}. The Fe sublattice of the compound order at 180 K in a cycloidal structure in the basal plane of the bct crystal structure. At 25 K the ordering of the Dy sublattice shows up. By the element specific technique of X-ray resonant magnetic scattering, the basal plane cycloidal structure was also found for the Dy sublattice. The work also includes neutron scattering studies of DyFe{sub 4}Al{sub 8} in magnetic fields up to 5 T applied along a <110> direction. The modulated structure at the Dy sublattice is quenched by a field lower than 1 T, whereas modulation is present at the Fe sublattice even when the 5 T field is applied. In the third part of the report, results from three small angle neutron experiments on MnSi are presented. At ambient pressure, a MnSi is known to form a helical spin density wave at temperature below 29 K. The application of 4.5 kbar pressure intended as hydrostatic decreased the Neel temperature to 25 K and changed the orientation of the modulation vector. To understand this reorientation within the current theoretical framework, anisotropic deformation of the sample crystal must be present. The development of magnetic critical scattering with an isotropic distribution of intensity has been studied at a level of detail higher than that of work found in the literature. Finally the potential of a novel polarization

  4. The nucleon axial mass and the MiniBooNE quasielastic neutrino-nucleus scattering problem

    International Nuclear Information System (INIS)

    Nieves, J.; Ruiz Simo, I.; Vicente Vacas, M.J.

    2012-01-01

    The charged-current double differential neutrino cross section, measured by the MiniBooNE Collaboration, has been analyzed using a microscopical model that accounts for, among other nuclear effects, long range nuclear (RPA) correlations and multinucleon scattering. We find that MiniBooNE data are fully compatible with the world average of the nucleon axial mass in contrast with several previous analyses which have suggested an anomalously large value. We also discuss the reliability of the algorithm used to estimate the neutrino energy.

  5. Neutron Inelastic Scattering Study of Liquid Argon

    Energy Technology Data Exchange (ETDEWEB)

    Skoeld, K; Rowe, J M; Ostrowski, G [Solid State Science Div., Argonne National Laboratory, Argonne, Illinois (US); Randolph, P D [Nuclear Technology Div., Idaho Nuclear Corporation, Idaho Falls, Idaho (US)

    1972-02-15

    The inelastic scattering functions for liquid argon have been measured at 85.2 K. The coherent scattering function was obtained from a measurement on pure A-36 and the incoherent function was derived from the result obtained from the A-36 sample and the result obtained from a mixture of A-36 and A-40 for which the scattering is predominantly incoherent. The data, which are presented as smooth scattering functions at constant values of the wave vector transfer in the range 10 - 44/nm, are corrected for multiple scattering contributions and for resolution effects. Such corrections are shown to be essential in the derivation of reliable scattering functions from neutron scattering data. The incoherent data are compared to recent molecular dynamics results and the mean square displacement as a function of time is derived. The coherent data are compared to molecular dynamics results and also, briefly, to some recent theoretical models

  6. Chiral symmetry restoration and quasi-elastic electron-nucleus scattering

    International Nuclear Information System (INIS)

    Henley, E.M.; Krein, G.

    1989-01-01

    Chiral symmetry is known to be an important concept in hadronic interactions. It holds in QCD, but is known to be broken at low energies. It is therefore useful to study chiral symmetry and its breaking together with its consequences in nuclear physics. It is the latter phenomena we consider here. It is difficult to study nonperturbative QCD at low energies and models are needed. The Nambu-Jona-Lasinio (NJL) model fits this category; it incorporates chiral symmetry and its breaking, and allows one to study its effects in nucleons and nuclei. In particular, the constituent quark mass varies with density (ρ) and temperature (T). At high ρ and T chiral symmetry is restored. It is the ρ dependence which yields important effects in electron scattering due to partial restoration of chiral symmetry in nuclei. We begin with the NJL model with a small chiral symmetry breaking

  7. The basic physics of neutron scattering experiments

    International Nuclear Information System (INIS)

    Mezei, F.

    1999-01-01

    The basic physical principles behind the well-established but also developing practice of neutron scattering experiments are presented. A few examples are given either to illustrate the physical principles or to give an idea of the variety, importance or magnitude of various phenomena. The evolution of neutron scattering experimental techniques is investigated from a special aspect: the increasing capability of taking into account more and more important and sometimes decisive finer details by using more and more realistic mathematical models of the evolution of the neutrons from birth do death, eventually passing by the sample and being scattered more than one times. Working with such numerical 'virtual instruments' one will have to go far beyond notions like resolution function, convolution etc, and actually eliminate a large number of approximations currently in use. (K.A.)

  8. Neutron Scattering and High Magnetic Fields

    Energy Technology Data Exchange (ETDEWEB)

    Winn, Barry L. [Oak Ridge National Lab. (ORNL), Oak Ridge, TN (United States); Stone, Matthew B. [Oak Ridge National Lab. (ORNL), Oak Ridge, TN (United States)

    2014-11-01

    The workshop “Neutron Scattering and High Magnetic Fields” was held September 4-5, 2014 at the Oak Ridge National Laboratory (ORNL). The workshop was held in response to a recent report by the National Research Council of the National Academy of Sciences entitled “High Magnetic Field Science and Its Application in the United States: Current Status and Future Directions.”1 This report highlights the fact that neutron scattering measurements carried out in high magnetic fields provide important opportunities for new science. The workshop explored the range of the scientific discoveries that could be enabled with neutron scattering measurements at high fields (25 Tesla or larger), the various technologies that might be utilized to build specialized instruments and sample environment equipment to enable this research at ORNL, and possible routes to funding and constructing these facilities and portable high field sample environments.

  9. Material classification by fast neutron scattering

    Energy Technology Data Exchange (ETDEWEB)

    Buffler, A. E-mail: abuffler@physci.uct.ac.za; Brooks, F.D. E-mail: brooks@physci.uct.ac.za; Allie, M.S.; Bharuth-Ram, K.; Nchodu, M.R

    2001-02-01

    The scattering of a beam of fast monoenergetic neutrons is used to determine elemental compositions of bulk samples (0.2-0.8 kg) of materials composed from one or more of the elements H, C, N, O, Al, S, Fe and Pb. Scattered neutrons are detected by liquid scintillators placed at forward and at backward angles. Different elements are identified by their characteristic scattering signatures derived either from a combination of time-of-flight and pulse height measurements, or from pulse height measurements alone. Scattering signatures measured for multi-element samples are analysed to determine atom fractions for H, C, N, O and other elements in the sample. Atom fractions determined from scattering signatures are insensitive to neutron interactions in material surrounding the scattering sample, provided the amount of material is not excessive. The atom fraction data are used to classify scattering material into categories including 'explosives', 'illicit drugs' and 'other materials' for the purpose of contraband detection.

  10. Influence of the effective mass of water molecule on thermal neutron scattering; Uticaj efektivne mase molekula vode na rasejanje termalnih neutrona

    Energy Technology Data Exchange (ETDEWEB)

    Markovic, M [Belgrade Univ. (Yugoslavia). Elektrotehnicki Fakultet

    1981-07-01

    The influence of the effective water molecule mass on the thermal neutron scattering on the nucleus of the hydrogen atom has been investigated. Besides the actual water molecule mass (M = 18) the investigations have been carried out with its two effective values (M1 = 16 and M2 = 20). The differential and total cross sections have been calculated for the incident thermal neutron energy E{sub o} = 1 eV. Investigation results show different prominence of the quantum effects and for M2 the appearance of peaks in the quasielastic scattering. (author)

  11. Quasielastic 3Hp and 3Hep scattering at intermediate energies and Glauber sum rules

    International Nuclear Information System (INIS)

    Blinov, A.V.; Vanyushin, I.A.; Grechko, V.E.

    1984-01-01

    Differential cross sections and average energy losses of fast protons in reactions p +3 H→psub(F)+X and p+ 3 He → psub(F)+X are studied making use of the ITEP liquid hydrogen bubble chamber of 80-cm diameter exposed to 2.5-GeV/c tritium nuclei (the kinetic energy of the incident protons in the nucleus rest frame Tsub(p)=0.318 GeV) and to 5-GeV/c 3 He nuclei (Tsub(p)=0.978 GeV). The experimental results are compared to predictions based on the sum rules for differential cross sections and average energy losses in the Glauber-Sitenko multiple scattering theory using the completeness condition for the wave functions of the nuclear excited states and the locality of the nuclear potential. The theory and the data are in good agreement at momentum of 2.5 GeV/c. Inconsistence between the Glauber sum rule predictions and the 5 GeV/c data is attributed to the Δ-isobar production in the intermediate state. It is found that possible six-quark bag admixture in the 3 H and 3 He nuclei does not exceed 5%

  12. Motility analysis of circularly swimming bull spermatozoa by quasi-elastic light scattering and cinematography.

    Science.gov (United States)

    Craig, T; Hallett, F R; Nickel, B

    1982-04-01

    The Rayleigh-Gans-Debye approximation is used to predict the electric field autocorrelation functions of light scattered from circularly swimming bull spermatozoa. Using parameters determined from cinematography and modeling the cells as coated ellipsoids of semiaxes a = 0.5 micrometers, b = 2.3 micrometers, and c = 9.0 micrometers, we were able to obtain model spectra that mimic the data exactly. A coat is found to be a necessary attribute of the particle. It is also clear that these model functions at 15 degrees may be represented by the relatively simple function used before by Hallett et al. (1978) to fit data from circularly swimming cells, thus giving some physical meaning to these functional shapes. Because of this agreement the half-widths of experimental functions can now be interpreted in terms of an oscillatory frequency for the movement of the circularly swimming cell. The cinematographic results show a trend to chaotic behavior as the temperature of the sample is increased, with concomitant decrease in overall efficiency. This is manifested by a decrease in oscillatory frequency and translational speed.

  13. Inelastic neutron scattering from glass formers

    International Nuclear Information System (INIS)

    Buchenau, U.

    1997-01-01

    Neutron spectra below and above the glass transition temperature show a pronounced difference between strong and fragile glass formers in Angell's fragility scheme. The strong anharmonic increase of the inelastic scattering with increasing temperature in fragile substances is absent in the strongest glass former SiO 2 . That difference is reflected in the temperature dependence of Brillouin sound velocities above the glass transition. Coherent inelastic neutron scattering data indicate a mixture of sound waves and local modes at the low frequency boson peak. A relation between the fragility and the temperature dependence of the transverse hypersound velocity at the glass temperature is derived. (author)

  14. Monte Carlo simulation of neutron scattering instruments

    International Nuclear Information System (INIS)

    Seeger, P.A.

    1995-01-01

    A library of Monte Carlo subroutines has been developed for the purpose of design of neutron scattering instruments. Using small-angle scattering as an example, the philosophy and structure of the library are described and the programs are used to compare instruments at continuous wave (CW) and long-pulse spallation source (LPSS) neutron facilities. The Monte Carlo results give a count-rate gain of a factor between 2 and 4 using time-of-flight analysis. This is comparable to scaling arguments based on the ratio of wavelength bandwidth to resolution width

  15. Analytic scattering kernels for neutron thermalization studies

    International Nuclear Information System (INIS)

    Sears, V.F.

    1990-01-01

    Current plans call for the inclusion of a liquid hydrogen or deuterium cold source in the NRU replacement vessel. This report is part of an ongoing study of neutron thermalization in such a cold source. Here, we develop a simple analytical model for the scattering kernel of monatomic and diatomic liquids. We also present the results of extensive numerical calculations based on this model for liquid hydrogen, liquid deuterium, and mixtures of the two. These calculations demonstrate the dependence of the scattering kernel on the incident and scattered-neutron energies, the behavior near rotational thresholds, the dependence on the centre-of-mass pair correlations, the dependence on the ortho concentration, and the dependence on the deuterium concentration in H 2 /D 2 mixtures. The total scattering cross sections are also calculated and compared with available experimental results

  16. Larmor-precession based neutron scattering instrumentation

    International Nuclear Information System (INIS)

    Ioffe, Alexander

    2009-01-01

    The Larmor precession of the neutron spin in a magnetic field allows the attachment of a Larmor clock to every neutron. Such Larmor labelling opens the possibility for the development of unusual neutron scattering techniques, where the energy (momentum) resolution does not require the initial and final states to be well selected. This principally allows for achievement of very high energy (momentum) resolution that is not feasible at all with conventional neutron scattering techniques, because the required neutron beam monochromatization (collimation) will result in intolerable intensity losses. Such decoupling of resolution and collimation allows, for example, for a significant increase in the luminosity of small-angle scattering or high-resolution diffractometers; the fact that opens new perspectives for their implementation at middle flux neutron sources. Different kinds of Larmor clock-based instrumentation, particularly two alternative NSE techniques using rotating and time-gradient magnetic field arrangements, which can be considered as inexpensive and affordable alternatives to present day NSE techniques, will be discussed and results of simulations and first experiments will be presented. (author)

  17. Small-angle neutron-scattering experiments

    International Nuclear Information System (INIS)

    Hardy, A.D.; Thomas, M.W.; Rouse, K.D.

    1981-04-01

    A brief introduction to the technique of small-angle neutron scattering is given. The layout and operation of the small-angle scattering spectrometer, mounted on the AERE PLUTO reactor, is also described. Results obtained using the spectrometer are presented for three materials (doped uranium dioxide, Magnox cladding and nitrided steel) of interest to Springfields Nuclear Power Development Laboratories. The results obtained are discussed in relation to other known data for these materials. (author)

  18. Dynamic neutron scattering from conformational dynamics. II. Application using molecular dynamics simulation and Markov modeling.

    Science.gov (United States)

    Yi, Zheng; Lindner, Benjamin; Prinz, Jan-Hendrik; Noé, Frank; Smith, Jeremy C

    2013-11-07

    Neutron scattering experiments directly probe the dynamics of complex molecules on the sub pico- to microsecond time scales. However, the assignment of the relaxations seen experimentally to specific structural rearrangements is difficult, since many of the underlying dynamical processes may exist on similar timescales. In an accompanying article, we present a theoretical approach to the analysis of molecular dynamics simulations with a Markov State Model (MSM) that permits the direct identification of structural transitions leading to each contributing relaxation process. Here, we demonstrate the use of the method by applying it to the configurational dynamics of the well-characterized alanine dipeptide. A practical procedure for deriving the MSM from an MD is introduced. The result is a 9-state MSM in the space of the backbone dihedral angles and the side-chain methyl group. The agreement between the quasielastic spectrum calculated directly from the atomic trajectories and that derived from the Markov state model is excellent. The dependence on the wavevector of the individual Markov processes is described. The procedure means that it is now practicable to interpret quasielastic scattering spectra in terms of well-defined intramolecular transitions with minimal a priori assumptions as to the nature of the dynamics taking place.

  19. Magnetism and magnetic materials probed with neutron scattering

    International Nuclear Information System (INIS)

    Velthuis, S.G.E. te; Pappas, C.

    2014-01-01

    Neutron scattering techniques are becoming increasingly accessible to a broader range of scientific communities, in part due to the onset of next-generation, high-power spallation sources, high-performance, sophisticated instruments and data analysis tools. These technical advances also advantageously impact research into magnetism and magnetic materials, where neutrons play a major role. In this Current Perspective series, the achievements and future prospects of elastic and inelastic neutron scattering, polarized neutron reflectometry, small angle neutron scattering, and neutron imaging, are highlighted as they apply to research into magnetic frustration, superconductivity and magnetism at the nanoscale. - Highlights: • Introduction to Current Perspective series titled Magnetism and Magnetic Materials probed with Neutron Scattering. • Elastic and inelastic neutron scattering in systems with magnetic frustration and superconductivity. • Small angle neutron scattering and polarized neutron reflectometry in studying magnetism at the nanoscale. • Imaging of magnetic fields and domains

  20. Magnetism and magnetic materials probed with neutron scattering

    Energy Technology Data Exchange (ETDEWEB)

    Velthuis, S.G.E. te, E-mail: tevelthuis@anl.gov [Materials Science Division, Argonne National Laboratory, 9700 S Cass Ave, Argonne, IL 60439 (United States); Pappas, C. [Faculty of Applied Sciences, Delft University of Technology, Mekelweg 15, NL-2629JB Delft (Netherlands)

    2014-01-15

    Neutron scattering techniques are becoming increasingly accessible to a broader range of scientific communities, in part due to the onset of next-generation, high-power spallation sources, high-performance, sophisticated instruments and data analysis tools. These technical advances also advantageously impact research into magnetism and magnetic materials, where neutrons play a major role. In this Current Perspective series, the achievements and future prospects of elastic and inelastic neutron scattering, polarized neutron reflectometry, small angle neutron scattering, and neutron imaging, are highlighted as they apply to research into magnetic frustration, superconductivity and magnetism at the nanoscale. - Highlights: • Introduction to Current Perspective series titled Magnetism and Magnetic Materials probed with Neutron Scattering. • Elastic and inelastic neutron scattering in systems with magnetic frustration and superconductivity. • Small angle neutron scattering and polarized neutron reflectometry in studying magnetism at the nanoscale. • Imaging of magnetic fields and domains.

  1. Interesting results from neutron-scattering

    International Nuclear Information System (INIS)

    Woods, A.D.B.

    Neutron scattering has been a useful tool in the determination of the lattice dynamics of metals, studies of the physics of magnetism in rare-earth systems, observing changes in the structure of DNA bases after ultraviolet irradiation, looking at plastic crystals, following structural phase changes in ferroelectric materials, and studying liquid He. Both low- and high-flux facilities are useful. (LL)

  2. Some applications of polarized inelastic neutron scattering

    Indian Academy of Sciences (India)

    A brief account of applications of polarized inelastic neutron scattering in condensed matter research is given. ... the itinerant antiferromagnet chromium we demonstrate that the dynamics of the longitudinal and transverse excitations are very different, resolving a long standing puzzle concerning the slope of their dispersion.

  3. Critical scattering of neutrons from terbium

    DEFF Research Database (Denmark)

    Als-Nielsen, Jens Aage; Dietrich, O.W.; Marshall, W.

    1968-01-01

    The inelasticity of the critical scattering of neutrons in terbium has been measured above the Neél temperature at the (0, 0, 2−Q) satellite position. The results show that dynamic slowing down of the fluctuations does occur in a second‐order phase transition in agreement with the general theory...

  4. NEUTRON-SCATTERING STUDY OF DCN

    DEFF Research Database (Denmark)

    Mackenzie, Gordon A.; Pawley, G. S.

    1979-01-01

    Phonons in deuterium cyanide have been measured by neutron coherent inelastic scattering. The main subject of study was the transverse acoustic mode in the (110) direction polarised along (110) which is associated with the first-order structural phase transition at 160K. Measurements have shown...

  5. Neutron scattering (progress report) January - December 1991

    International Nuclear Information System (INIS)

    Buehrer, W.; Fischer, P.; Furrer, A.

    1992-02-01

    Progress made by the Laboratory for Neutron Scattering of the Swiss Federal Institute of Technology during the year 1991 in the fields of high-T c superconductors, materials science, magnetism, structural research, lattice dynamics, phase transitions, instrumental and support activities is reported. figs., tabs., refs

  6. Experimental technique of small angle neutron scattering

    International Nuclear Information System (INIS)

    Xia Qingzhong; Chen Bo

    2006-03-01

    The main parts of Small Angle Neutron Scattering (SANS) spectrometer, and their function and different parameters are introduced from experimental aspect. Detailed information is also introduced for SANS spectrometer 'Membrana-2'. Based on practical experiments, the fundamental requirements and working condition for SANS experiments, including sample preparation, detector calibration, standard sample selection and data preliminary process are described. (authors)

  7. Neutron elastic scattering at very small angles

    CERN Multimedia

    2002-01-01

    This experiment will measure neutron-proton elastic scattering at very small angles and hence very small four-momentum transfer, |t|. The range of |t| depends on the incident neutron momentum of the events but the geometrical acceptance will cover the angular range 0.025 < $\\Theta_{lab}$ < 1.9 mrad. The higher figure could be extended to 8.4 mrad by changing the geometry of the experiment in a later phase. \\\\ \\\\ The neutron beam will be highly collimated and will be derived from a 400 GeV external proton beam of up to $4 \\times 10^{10}$ protons per pulse in the SPS North Area Hall 1. The hydrogen target will be gaseous, operating at 40 atm. pressure and acts as a multiwire proportional chamber to detect the recoil protons. The forward neutron will be detected and located by interaction in a neutron vertex detector and its energy measured by a conventional steel plate calorimeter. \\\\ \\\\ The experiment will cover the angular region of nucleon-nucleon scattering which is dominated by Coulomb scattering ...

  8. Resonance effects in neutron scattering lengths

    Energy Technology Data Exchange (ETDEWEB)

    Lynn, J.E.

    1989-06-01

    The nature of neutron scattering lengths is described and the nuclear effects giving rise to their variation is discussed. Some examples of the shortcomings of the available nuclear data base, particularly for heavy nuclei, are given. Methods are presented for improving this data base, in particular for obtaining the energy variation of the complex coherent scattering length from long to sub-/angstrom/ wave lengths from the available sources of slow neutron cross section data. Examples of this information are given for several of the rare earth nuclides. Some examples of the effect of resonances in neutron reflection and diffraction are discussed. This report documents a seminar given at Argonne National Laboratory in March 1989. 18 refs., 18 figs.

  9. 2016 American Conference on Neutron Scattering (ACNS)

    International Nuclear Information System (INIS)

    Woodward, Patrick

    2017-01-01

    The 8th American Conference on Neutron Scattering (ACNS) was held July 10-14, 2016 in Long Beach California, marking the first time the meeting has been held on the west coast. The meeting was coordinated by the Neutron Scattering Society of America (NSSA), and attracted 285 attendees. The meeting was chaired by NSSA vice president Patrick Woodward (the Ohio State University) assisted by NSSA president Stephan Rosenkranz (Argonne National Laboratory) together with the local organizing chair, Brent Fultz (California Institute of Technology). As in past years the Materials Research Society assisted with planning, logistics and operation of the conference. The science program was divided into the following research areas: (a) Sources, Instrumentation, and Software; (b) Hard Condensed Matter; (c) Soft Matter; (d) Biology; (e) Materials Chemistry and Materials for Energy; (f) Engineering and Industrial Applications; and (g) Neutron Physics.

  10. Fast neutron scattering near shell closures: Scandium

    International Nuclear Information System (INIS)

    Smith, A.B.; Guenther, P.T.

    1992-08-01

    Neutron differential elastic- and inelastic-scattering cross sections are measured from ∼ 1.5 to 10 MeV with sufficient detail to define the energy-averaged behavior of the scattering processes. Neutrons corresponding to excitations of 465 ± 23, 737 ± 20, 1017 ± 34, 1251 ± 20, 1432 ± 23 and 1692 ± 25 keV are observed. It is shown that the observables, including the absorption cross section, are reasonably described with a conventional optical-statistical model having energy-dependent geometric parameters. These energy dependencies are alleviated when the model is extended to include the contributions of the dispersion relationship. The model parameters are conventional, with no indication of anomalous behavior of the neutron interaction with 45 Sc, five nucleons from the doubly closed shell at 40 Ca

  11. Resonance effects in neutron scattering lengths

    International Nuclear Information System (INIS)

    Lynn, J.E.

    1989-01-01

    The nature of neutron scattering lengths is described and the nuclear effects giving rise to their variation is discussed. Some examples of the shortcomings of the available nuclear data base, particularly for heavy nuclei, are given. Methods are presented for improving this data base, in particular for obtaining the energy variation of the complex coherent scattering length from long to sub-angstrom wave lengths from the available sources of slow neutron cross section data. Examples of this information are given for several of the rare earth nuclides. Some examples of the effect of resonances in neutron reflection and diffraction are discussed. This report documents a seminar given at Argonne National Laboratory in March 1989. 18 refs., 18 figs

  12. 2016 American Conference on Neutron Scattering (ACNS)

    Energy Technology Data Exchange (ETDEWEB)

    Woodward, Patrick [Materials Research Society, Warrendale, PA (United States)

    2017-02-09

    The 8th American Conference on Neutron Scattering (ACNS) was held July 10-14, 2016 in Long Beach California, marking the first time the meeting has been held on the west coast. The meeting was coordinated by the Neutron Scattering Society of America (NSSA), and attracted 285 attendees. The meeting was chaired by NSSA vice president Patrick Woodward (the Ohio State University) assisted by NSSA president Stephan Rosenkranz (Argonne National Laboratory) together with the local organizing chair, Brent Fultz (California Institute of Technology). As in past years the Materials Research Society assisted with planning, logistics and operation of the conference. The science program was divided into the following research areas: (a) Sources, Instrumentation, and Software; (b) Hard Condensed Matter; (c) Soft Matter; (d) Biology; (e) Materials Chemistry and Materials for Energy; (f) Engineering and Industrial Applications; and (g) Neutron Physics.

  13. Quantum entanglement and neutron scattering experiments

    International Nuclear Information System (INIS)

    Cowley, R A

    2003-01-01

    It is shown that quantum entanglement in condensed matter can be observed with scattering experiments if the energy resolution of the experiments enables a clear separation between the elastic scattering and the scattering from the excitations in the system. These conditions are not satisfied in recent deep inelastic neutron scattering experiments from hydrogen-containing systems that have been interpreted as showing the existence of quantum entanglement for short times in, for example, water at room temperature. It is shown that the theory put forward to explain these experiments is inconsistent with the first-moment sum rule for the Van Hove scattering function and we suggest that the theory is incorrect. The experiments were performed using the unique EVS spectrometer at ISIS and suggestions are made about how the data and their interpretation should be re-examined

  14. Neutron scattering study of dilute supercritical solutions

    International Nuclear Information System (INIS)

    Cochran, H.D.; Wignall, G.D.; Shah, V.M.; Londono, J.D.; Bienkowski, P.R.

    1994-01-01

    Dilute solutions in supercritical solvents exhibit interesting microstructures that are related to their dramatic macroscopic behavior. In typical attractive solutions, solutes are believed to be surrounded by clusters of solvent molecules, and solute molecules are believed to congregate in the vicinity of one another. Repulsive solutions, on the other hand, exhibit a local region of reduced solvent density around the solute with solute-solute congregation. Such microstructures influence solubility, partial molar volume, reaction kinetics, and many other properties. We have undertaken to observe these interesting microstructures directly by neutron scattering experiments on dilute noble gas systems including Ar. The three partial structure factors for such systems and the corresponding pair correlation functions can be determined by using the isotope substitution technique. The systems studied are uniquely suited for our objectives because of the large coherent neutron scattering length of the isotope 36 Ar and because of the accurate potential energy functions that are available for use in molecular simulations and theoretical calculations to be compared with the scattering results. We will describe our experiment, the unique apparatus we have built for it, and the neutron scattering results from our initial allocations of beam time. We will also describe planned scattering experiments to follow those with noble gases, including study of long-chain molecules in supercritical solvents. Such studies will involve hydrocarbon mixtures with and without deuteration to provide contrast

  15. The Manuel Lujan Jr. Neutron Scattering Center

    International Nuclear Information System (INIS)

    Goldstone, J.A.

    1994-01-01

    High in the northcentral mountains of Los Alamos, New Mexico, is the Manuel Lujan Jr. Neutron Scattering Center (LANSCE), a pulsed-spallation neutron source located at Los Alamos National Laboratory. At LANSCE, neutrons are produced by spallation when a pulsed 800-MeV proton beam impinges on a tungsten target. The proton pulses are provided by a linear accelerator and an associated Proton Storage Ring (PSR), which alters the intensity, time structure, and repetition rate of the pulses. In October 1986, LANSCE was designated a national user facility, with a formal user program initiated in 1988. In July 1989, the LANSCE facility was dedicated as the Manuel Lujan Jr. Neutron Scattering Center in honor of the long-term Congressman from New Mexico. At present, the PSR operates with a proton pulse width of 0.27 μs at 20 Hz and 80 μA, attaining the highest peak neutron flux in the world and close to its goal of 100 μA, which would yield a peak thermal neutron flux of 10 16 n/cm -2 s -1 . This paper discusses the target/moderator/reflector shield system, the LANSCE instruments, the facility improvement projects, and user programs

  16. [Gamma scattering in condensed matter with high intensity Moessbauer radiation

    International Nuclear Information System (INIS)

    1992-01-01

    This report discusses: quasielastic scattering studies on glycerol; gamma-ray scattering from alkali halides; lattice dynamics in metals; Moessbauer neutron scattering, x-ray diffraction, and macroscopic studies of high T c superconductors containing tungsten; NiAl scattering studies; and atomic interference factors and nuclear Casimir effect

  17. An automated analysis workflow for optimization of force-field parameters using neutron scattering data

    Energy Technology Data Exchange (ETDEWEB)

    Lynch, Vickie E.; Borreguero, Jose M. [Neutron Data Analysis & Visualization Division, Oak Ridge National Laboratory, Oak Ridge, TN, 37831 (United States); Bhowmik, Debsindhu [Computational Sciences & Engineering Division, Oak Ridge National Laboratory, Oak Ridge, TN, 37831 (United States); Ganesh, Panchapakesan; Sumpter, Bobby G. [Center for Nanophase Material Sciences, Oak Ridge National Laboratory, Oak Ridge, TN, 37831 (United States); Computational Sciences & Engineering Division, Oak Ridge National Laboratory, Oak Ridge, TN, 37831 (United States); Proffen, Thomas E. [Neutron Data Analysis & Visualization Division, Oak Ridge National Laboratory, Oak Ridge, TN, 37831 (United States); Goswami, Monojoy, E-mail: goswamim@ornl.gov [Center for Nanophase Material Sciences, Oak Ridge National Laboratory, Oak Ridge, TN, 37831 (United States); Computational Sciences & Engineering Division, Oak Ridge National Laboratory, Oak Ridge, TN, 37831 (United States)

    2017-07-01

    Graphical abstract: - Highlights: • An automated workflow to optimize force-field parameters. • Used the workflow to optimize force-field parameter for a system containing nanodiamond and tRNA. • The mechanism relies on molecular dynamics simulation and neutron scattering experimental data. • The workflow can be generalized to any other experimental and simulation techniques. - Abstract: Large-scale simulations and data analysis are often required to explain neutron scattering experiments to establish a connection between the fundamental physics at the nanoscale and data probed by neutrons. However, to perform simulations at experimental conditions it is critical to use correct force-field (FF) parameters which are unfortunately not available for most complex experimental systems. In this work, we have developed a workflow optimization technique to provide optimized FF parameters by comparing molecular dynamics (MD) to neutron scattering data. We describe the workflow in detail by using an example system consisting of tRNA and hydrophilic nanodiamonds in a deuterated water (D{sub 2}O) environment. Quasi-elastic neutron scattering (QENS) data show a faster motion of the tRNA in the presence of nanodiamond than without the ND. To compare the QENS and MD results quantitatively, a proper choice of FF parameters is necessary. We use an efficient workflow to optimize the FF parameters between the hydrophilic nanodiamond and water by comparing to the QENS data. Our results show that we can obtain accurate FF parameters by using this technique. The workflow can be generalized to other types of neutron data for FF optimization, such as vibrational spectroscopy and spin echo.

  18. Measurement of the muon antineutrino double-differential cross section for quasielastic-like scattering on hydrocarbon at Eν˜3.5 GeV

    Science.gov (United States)

    Patrick, C. E.; Aliaga, L.; Bashyal, A.; Bellantoni, L.; Bercellie, A.; Betancourt, M.; Bodek, A.; Bravar, A.; Budd, H.; Caceres v., G. F. R.; Carneiro, M. F.; Chavarria, E.; da Motta, H.; Dytman, S. A.; Díaz, G. A.; Felix, J.; Fields, L.; Fine, R.; Gago, A. M.; Galindo, R.; Gallagher, H.; Ghosh, A.; Gran, R.; Han, J. Y.; Harris, D. A.; Henry, S.; Hurtado, K.; Jena, D.; Kleykamp, J.; Kordosky, M.; Le, T.; Lu, X.-G.; Maher, E.; Manly, S.; Mann, W. A.; Marshall, C. M.; McFarland, K. S.; McGowan, A. M.; Messerly, B.; Miller, J.; Mislivec, A.; Morfín, J. G.; Mousseau, J.; Naples, D.; Nelson, J. K.; Norrick, A.; Nowak, G. M.; Nuruzzaman, Paolone, V.; Perdue, G. N.; Peters, E.; Ramírez, M. A.; Ransome, R. D.; Ray, H.; Ren, L.; Rodrigues, P. A.; Ruterbories, D.; Schellman, H.; Solano Salinas, C. J.; Sultana, M.; Sánchez Falero, S.; Teklu, A. M.; Valencia, E.; Wolcott, J.; Wospakrik, M.; Yaeggy, B.; Zhang, D.; Miner ν A Collaboration

    2018-03-01

    We present double-differential measurements of antineutrino charged-current quasielastic scattering in the MINERvA detector. This study improves on a previous single-differential measurement by using updated reconstruction algorithms and interaction models and provides a complete description of observed muon kinematics in the form of a double-differential cross section with respect to muon transverse and longitudinal momentum. We include in our signal definition zero-meson final states arising from multinucleon interactions and from resonant pion production followed by pion absorption in the primary nucleus. We find that model agreement is considerably improved by a model tuned to MINERvA inclusive neutrino scattering data that incorporates nuclear effects such as weak nuclear screening and two-particle, two-hole enhancements.

  19. Neutron scattering on deformed nuclei

    International Nuclear Information System (INIS)

    Hansen, L.F.; Haight, R.C.; Pohl, B.A.; Wong, C.; Lagrange, C.

    1984-09-01

    Measurements of neutron elastic and inelastic differential cross sections around 14 MeV for 9 Be, C, 181 Ta, 232 Th, 238 U and 239 Pu have been analyzed using a coupled channel (CC) formalism for deformed nuclei and phenomenological global optical model potentials (OMP). For the actinide targets these results are compared with the predictions of a semi-microscopic calculation using Jeukenne, Lejeune and Mahaux (JLM) microscopic OMP and a deformed ground state nuclear density. The overall agreement between calculations and the measurements is reasonable good even for the very light nuclei, where the quality of the fits is better than those obtained with spherical OMP

  20. Neutron transfer with anisotropic scattering

    International Nuclear Information System (INIS)

    El Wakil, S.A.; Haggag, M.H.; Saad, E.A.

    1979-01-01

    The finite slab problem is reduced to a semi-infinite one by adding an infinitesimally thick layer such that both the added layer and the total layer are semi-infinite. The relation between the reflection and transmission functions for a finite slab and those for an infinite one are obtained in terms of an operator which satisfies a semigroup equation. The method is applied to anisotropic scattering with azimuthal dependence. Numerical calculations are made and the results compared with those of other workers. (author)

  1. Properties of thermal neutron scattering on the nucleus of hydrogen atom of methane molecule; Osobine rasejanja termalnih neutrona na jezgru vodonikovog atoma molekula metana

    Energy Technology Data Exchange (ETDEWEB)

    Miloradovic, M M [Tehnicki fakultet, Cacak (Yugoslavia); Markovic, M I [Elektrotehnicki fakultet, Beograd (Yugoslavia)

    1987-07-01

    On the basis of derived quantum-mechanical expression for the microscopic nucleus scattering the single and collective influences of translational, rotational and intravibrational motions of the methane molecule on the thermal neutron scattering are established. When incident neutron energy is E{sub 0} {<=} 0.1 eV, it is found that only translational and rotational motion of the methane molecule influences the thermal neutron scattering. The influence of these motions for E{sub 0} . 0.1 eV decreases rapidly with the increase of the incident neutron energy and then the significant influence on the thermal neutron scattering exerts inelastic scattering on the combined rotational with single intravibrational phonons of the methane molecule, while the inelastic scattering on single intravibrational phonons is significantly less. In the combination with rotational phonons the biggest influence has threefold degenerated deformed intravibrational phonons, somehow less influence has twofold degenerated deformed intravibrational phonons, and the least influence has valent intravibrational phonons. All the effects of quasielastic and quantum inelastic scattering are clearly expressed with the thermal neutron scattering at small angles, so that for E{sub 0} =1 eV practically there is no scattering backward. (author)

  2. Proceedings of the workshop on neutron scattering instrumentation for SNQ

    International Nuclear Information System (INIS)

    Scherm, R.; Stiller, H.

    1984-10-01

    These proceedings contain the articles presented at the named workshop. These concern instrumentation for neutron diffraction with special regards to small angle scattering, diffuse scattering, inelastic scattering, high resolution spectroscopy, and special techniques. (HSI)

  3. Quasielastic reactions

    International Nuclear Information System (INIS)

    Henning, W.

    1979-01-01

    Quasielastic reaction studies, because of their capability to microscopically probe nuclear structure, are still of considerable interest in heavy-ion reactions. The recent progress in understanding various aspects of the reaction mechanism make this aim appear closer. The relation between microscopic and macroscopic behavior, as suggested, for example, by the single proton transfer data to individual final states or averaged excitation energy intervals, needs to be explored. It seems particularly useful to extend measurements to higher incident energies, to explore and understand nuclear structure aspects up to the limit of the energy range where they are important

  4. Theory of neutron scattering in disordered alloys

    International Nuclear Information System (INIS)

    Yussouff, M.; Mookerjee, A.

    1984-08-01

    A comprehensive theory of thermal neutron scattering in disordered alloys is presented here. We consider in detail the case of substitutional random binary alloy with random changes in mass and force constants; and for all values of the concentration. The cluster CPA formalism in argumented space developed here is free from analytical difficulties for the Green function, performs correct averaging over random atomic scattering lengths and employs a self-consistent medium for the calculations. For easy computation, we describe the graphical representation of the resolvent where the approximation steps can be depicted as closed paths in augmented space. Our results for scattering cross sections, both coherent and incoherent, include new types of terms and these lead to asymmetric line shapes for the coherent scattering. (author)

  5. Scattering of fast neutrons from 103Rh

    International Nuclear Information System (INIS)

    Barnard, E.; Reitmann, D.

    1978-01-01

    The scattering of fast neutrons from 103 Rh was studied by means of (n, n), (n, n') and (n, n'γ) measurements at neutron energies up to 2 MeV. More than fifty unknown γ-transitions were identified and a level scheme established which includes fifteen unreported excited states. Branching ratios, spins and parities for these levels were deduced, as well as the effective activation cross sections for the 103 Rh(n, n')sup(103m)Rh reaction. The results are compared with existing data and with calculations based on the optical and statistical models. (Auth.)

  6. A mechanical rotator for neutron scattering measurements

    International Nuclear Information System (INIS)

    Thaler, A.; Northen, E.; Aczel, A. A.; MacDougall, G. J.

    2016-01-01

    We have designed and built a mechanical rotation system for use in single crystal neutron scattering experiments at low temperatures. The main motivation for this device is to facilitate the application of magnetic fields transverse to a primary training axis, using only a vertical cryomagnet. Development was done in the context of a triple-axis neutron spectrometer, but the design is such that it can be generalized to a number of different instruments or measurement techniques. Here, we discuss some of the experimental constraints motivating the design, followed by design specifics, preliminary experimental results, and a discussion of potential uses and future extension possibilities.

  7. A Precision Measurement of the Transverse Asymmetry AT from Quasi-elastic 3He(e,e') process, and the Neutron Magnetic Form Factor GNM at low Q2

    Energy Technology Data Exchange (ETDEWEB)

    Xu, Wang [Massachusetts Inst. of Technology (MIT), Cambridge, MA (United States)

    2002-06-01

    Electromagnetic form factors are fundamental quantities in describing the underlying electromagnetic structure of nucleons. While proton electromagnetic form factors have been determined with good precision, neutron form factors are known poorly, largely due to the lack of free neutron targets. Jefferson Lab Hall A experiment E95-001, a ''precise measurement of the transverse asymmetry AT' from the quasielastic 3He(e, e') process,'' was therefore designed to determine precisely the neutron magnetic form factor, G$n\\atop{M}$ at low momentum transfer values and was successfully completed in Spring 1999. High precision AT'data in the quasi-elastic region at Q2 values of 0.1 to 0.6 (GeV/c)2 were obtained using a high-pressure spin-exchange optically-pumped polarized 3He gas target with an average polarization of 30%, a longitudinally polarized e- beam, and two High Resolution Spectrometers: HRSe and HRSh. HRSe was employed to detect scattered electrons from the quasi-elastic kinematic region, and HRSh was employed as a elastic polarimetry to monitor the product of the beam and target polarizations. The extraction of form factors is usually model-dependent. Significant constraints on theoretical calculations are provided bu additional high precision quasi-elastic asymmetry data at Q2 values of 0.1 and 0.2 (GeV/c)2 in 3He breakup region, where effects of final state interactions (FSI) and meson exchange currents (MEC) are expected to be large [71]. G$n\\atop{M}$ is extracted from a non-relativistic Faddeev calculation which includes both FSI and MEC at Q2 values of 0.1 and 0.2 (GeV/c)2. The uncertainties of G$n\\atop{M}$ at these Q2 values are comparable to those of recent experiments with deuterium targets [58]. At the higher Q2 values from this experiment, G$n\\atop{M}$ is extracted

  8. Neutron-scattering studies of the S=2 antiferromagnetic chain MnCl sub 3 (C sub 1 sub 0 D sub 8 N sub 2)

    CERN Document Server

    Granroth, G E; Coldea, R; Eccleston, R S; Ward, B H; Talham, D R; Meisel, M W

    2002-01-01

    Quasi-elastic and inelastic neutron scattering studies of the quasi-one-dimensional S=2 antiferromagnet MnCl sub 3 (C sub 1 sub 0 D sub 8 N sub 2) are reported. The quasi-elastic measurements exhibit a broad peak at Q approx 0.69 A sup - sup 1 , which is consistent with short-range antiferromagnetic coupling between neighboring Mn sup 3 sup + ions. Inelastic experiments, at 150 mK and Q=0.70 A sup - sup 1 , reveal decreased magnetic scattering at energies less than 0.2 meV when compared to similar studies at 20 K. These results provide microscopic evidence for the presence of a Haldane gap and are consistent with the bulk magnetization measurements of Granroth et al. (orig.)

  9. Neutron scattering from polarised proton domains

    CERN Document Server

    Van den Brandt, B; Kohbrecher, J; Konter, J A; Mango, S; Glattli, H; Leymarie, E; Grillo, I; May, R P; Jouve, H; Stuhrmann, H B; Stuhrmann, H B; Zimmer, O

    2002-01-01

    Time-dependent small-angle polarised neutron scattering from domains of polarised protons has been observed at the onset of dynamic nuclear polarisation in a frozen solution of 98% deuterated glycerol-water at 1 K containing a small concentration of paramagnetic centres (EHBA-Cr sup V). Simultaneous NMR measurements show that the observed scattering arises from protons around the Cr sup V -ions which are polarised to approx 10% in a few seconds, much faster than the protons in the bulk. (authors)

  10. Neutron scattering. Annual progress report 1997

    International Nuclear Information System (INIS)

    Allenspach, P.; Boeni, B.; Fischer, P.; Furrer, A.

    1998-02-01

    The present progress report describes the scientific and technical activities obtained by LNS staff members in 1997. It also includes the work performed by external groups at our CRG instruments D1A and IN3 at the ILL Grenoble. Due to the outstanding properties of neutrons and x-rays the research work covered many areas of science and materials research. The highlight of the year 1997 was certainly the production of neutrons at the new spallation neutron source SINQ. From July to November, SINQ was operating for typically two days/week and allowed the commissioning of four instruments at the neutron guide system: - the triple-axis spectrometer Druechal, - the powder diffractometer DMC, - the double-axis diffractometer TOPSI, the polarised triple-axis spectrometer TASP. These instruments are now fully operational and have already been used for condensed matter studies, partly in cooperation with external groups. Five further instruments are in an advanced state, and their commissioning is expected to occur between June and October 1998: - the high-resolution powder diffractometer HRPT, - the single-crystal diffractometer TriCS, - the time-of-flight spectrometer FOCUS, - the reflectometer AMOR, - the neutron optical bench NOB. Together with the small angle neutron scattering facility SANS operated by the spallation source department, all these instruments will be made available to external user groups in the future. (author) figs., tabs., refs

  11. Specimen environments in thermal neutron scattering experiments

    International Nuclear Information System (INIS)

    Cebula, D.J.

    1980-11-01

    This report is an attempt to collect into one place outline information concerning the techniques used and basic design of sample environment apparatus employed in neutron scattering experiments. Preliminary recommendations for the specimen environment programme of the SNS are presented. The general conclusion reached is that effort should be devoted towards improving reliability and efficiency of operation of specimen environment apparatus and developing systems which are robust and easy to use, rather than achieving performance at the limits of technology. (author)

  12. Summary of coherent neutron scattering length

    International Nuclear Information System (INIS)

    Rauch, H.

    1981-07-01

    Experimental values of neutron-nuclei bound scattering lengths for some 354 isotopes and elements and the various spin-states are compiled in a uniform way together with their error bars as quoted in the original literature. Recommended values are also given. The definitions of the relevant quantities presented in the data tables and the basic principles of measurements are explained in the introductory chapters. The data is also available on a magnetic tape

  13. Monte Carlo simulation of neutron scattering instruments

    International Nuclear Information System (INIS)

    Seeger, P.A.; Daemen, L.L.; Hjelm, R.P. Jr.

    1998-01-01

    A code package consisting of the Monte Carlo Library MCLIB, the executing code MC RUN, the web application MC Web, and various ancillary codes is proposed as an open standard for simulation of neutron scattering instruments. The architecture of the package includes structures to define surfaces, regions, and optical elements contained in regions. A particle is defined by its vector position and velocity, its time of flight, its mass and charge, and a polarization vector. The MC RUN code handles neutron transport and bookkeeping, while the action on the neutron within any region is computed using algorithms that may be deterministic, probabilistic, or a combination. Complete versatility is possible because the existing library may be supplemented by any procedures a user is able to code. Some examples are shown

  14. Neutron scattering studies of Mn12-acetate

    International Nuclear Information System (INIS)

    Robinson, R.A.

    2000-01-01

    Full text: The S=10 magnetic molecule Mn 12 -acetate, which crystallises into a tetragonal crystal structure, has attracted substantial recent attention by virtue of its low temperature bulk magnetic properties, which give evidence for resonant quantum tunnelling of the magnetisation. We report a full neutron crystal structure including positions of all protons/deuterons, including the solvated water and acetic acid, a polarised-neutron study of the real space magnetisation, which confirms a simple magnetic-structure model for the molecule, albeit with reduced Mn moments, and inelastic neutron scattering data containing both the excitations within the 21-fold degenerate S=10 manifold, and those from S=10 to the S=9 manifolds. Both manifolds are split by uniaxial magnetic anisotropy, and we report coefficients for 2nd and 4th-order terms in the magnetic Hamiltonian

  15. Neutron scattering studies on frustrated magnets

    International Nuclear Information System (INIS)

    Arima, Taka-hisa

    2013-01-01

    A lot of frustrated magnetic systems exhibit a nontrivial magnetic order, such as long-wavelength modulation, noncollinear, or noncoplanar order. The nontrivial order may pave the way for the novel magnetic function of matter. Neutron studies are necessary to determine the magnetic structures in the frustrated magnetic systems. In particular, spin-polarized neutron scattering is a useful technique for the investigation of the novel physical properties relevant to the nontrivial spin arrangement. Here some neutron studies on a multiferroic perovskite manganese oxide system are demonstrated as a typical case. The frustrated magnetic systems may also a playground of novel types of local magnetic excitations, which behave like particles in contrast to the magnetic waves. It is becoming a good challenge to study such particle-type magnetic excitations relevant to the magnetic frustration. (author)

  16. Neutron scattering cross sections of uranium-238

    International Nuclear Information System (INIS)

    Beghian, L.E.; Kegel, G.H.R.; Marcella, T.V.; Barnes, B.K.; Couchell, G.P.; Egan, J.J.; Mittler, A.; Pullen, D.J.; Schier, W.A.

    1979-01-01

    The University of Lowell high-resolution time-of-flight spectrometer was used to measure angular distributions and 90-deg excitation functions for neutrons scattered from 238 U in the energy range from 0.9 to 3.1 MeV. This study was limited to the elastic and the first two inelastic groups, corresponding to states of 238 U at 45 keV (2 + ) and 148 keV (4 + ). Angular distributions were measured at primary neutron energies of 1.1, 1.9, 2.5, and 3.1 MeV for the same three neutron groups. Whereas the elastic data are in fair agreement with the evaluation in the ENDF/B-IV file, there is substantial disagreement between the inelastic measurements and the evaluated cross sections. 12 figures

  17. Study of material science by neutron scattering

    International Nuclear Information System (INIS)

    Kim, H.J.; Yoon, B.K.; Cheon, B.C.; Lee, C.Y.; Kim, C.S.

    1980-01-01

    To develop accurate methods of texture measurement in metallic materials by neutron diffraction, (100),(200),(111) and (310) pole figures have been measured for the oriented silicon steel sheet, and currently study of correction methods for neutron absorption and extinction effects are in progress. For quantitative analysis of texture of polycrystalline material with a cubic structure, a software has been developed to calculate inverse pole figures for arbitrary direction specified in the speciman as well as pole figures for arbitrary chosen crystallographic planes from three experimental pole figures. This work is to be extended for the calculation of three dimensional orientation distribution function and for the evaluation of errors in the quantitative analysis of texture. Work is also for the study of N-H...O hydrogen bond in amino acid by observing molecular motions using neutron inelastic scattering. Measurement of neutron inelastic scattering spectrum of L-Serine is completed at 100 0 K and over the energy transfer range of 20-150 meV. (KAERI INIS Section)

  18. Spectral distortion due to scattered cold neutrons in beryllium filter

    International Nuclear Information System (INIS)

    Sakamoto, Yukio; Inoue, Kazuhiko

    1980-01-01

    Polycrystalline beryllium filters are used to discriminate the cold neutrons from the thermal neutrons with energies above Bragg cut-off energy. The cold neutron scattering cross section is very small, but the remaining cross section is not zero. Then the neutrons scattered once from the filter in the cold neutron energy region have chance of impinging on the outlet of filter. Those neutrons are almost upscattered and develop into thermal neutrons; thus the discriminated cold neutrons include a small spectral distortion due to the thermal neutrons. In the present work we have evaluated the effect on the cold neutron spectrum due to the repeatedly scattered and transmitted neutrons by using a Monte Carlo calculation method. (author)

  19. A neutron scattering study of DCN

    International Nuclear Information System (INIS)

    Mackenzie, G.A.; Pawley, G.S.

    1979-01-01

    Phonons in deuterium cyanide have been measured by neutron coherent inelastic scattering. The main subject of study was the transverse acoustic mode in the (110) direction polarised along (110) which is associated with the first-order structural phase transition at 160 K. Measurements have shown that the frequency decreases by about 25% between about 225 and 160 K as the transition temperature is approached. The other acoustic modes observable in the a*b* scattering plane have been measured and show no anomalous temperature dependence. Optic modes were unobservable because of the small size of the single-crystal sample which gave insufficient scattered intensity. Apart from the 'soft' mode, the measured frequencies are in good agreement with lattice dynamics calculations. (author)

  20. Development of temperature related thermal neutron scattering database for MCNP

    International Nuclear Information System (INIS)

    Mei Longwei; Cai Xiangzhou; Jiang Dazhen; Chen Jingen; Guo Wei

    2013-01-01

    Based on ENDF/B-Ⅶ neutron library, the thermal neutron scattering library S(α, β) for molten salt reactor moderators was developed. The temperatures of this library were chose as the characteristic temperature of the molten salt reactor. The cross section of the thermal neutron scattering of ACE format was investigated, and this library was also validated by the benchmarks of ICSBEP. The uncertainties shown in the validation were in reasonable range when compared with the thermal neutron scattering library tmccs which included in the MCNP data library. It was proved that the thermal neutron scattering library processed in this study could be used in the molten salt reactor design. (authors)

  1. Neutron scattering applications in structural biology: now and the future

    Energy Technology Data Exchange (ETDEWEB)

    Trewhella, J [Los Alamos National Lab., NM (United States)

    1996-05-01

    Neutrons have an important role to play in structural biology. Neutron crystallography, small-angle neutron scattering and inelastic neutron scattering techniques all contribute unique information on biomolecular structures. In particular, solution scattering techniques give critical information on the conformations and dispositions of the components of complex assemblies under a wide variety of relevant conditions. The power of these methods is demonstrated here by studies of protein/DNA complexes, and Ca{sup 2+}-binding proteins complexed with their regulatory targets. In addition, we demonstrate the utility of a new structural approach using neutron resonance scattering. The impact of biological neutron scattering to date has been constrained principally by the available fluxes at neutron sources and the true potential of these approaches will only be realized with the development of new more powerful neutron sources. (author)

  2. New evaluation of thermal neutron scattering libraries for light and heavy water

    Directory of Open Access Journals (Sweden)

    Marquez Damian Jose Ignacio

    2017-01-01

    Full Text Available In order to improve the design and safety of thermal nuclear reactors and for verification of criticality safety conditions on systems with significant amount of fissile materials and water, it is necessary to perform high-precision neutron transport calculations and estimate uncertainties of the results. These calculations are based on neutron interaction data distributed in evaluated nuclear data libraries. To improve the evaluations of thermal scattering sub-libraries, we developed a set of thermal neutron scattering cross sections (scattering kernels for hydrogen bound in light water, and deuterium and oxygen bound in heavy water, in the ENDF-6 format from room temperature up to the critical temperatures of molecular liquids. The new evaluations were generated and processable with NJOY99 and also with NJOY-2012 with minor modifications (updates, and with the new version of NJOY-2016. The new TSL libraries are based on molecular dynamics simulations with GROMACS and recent experimental data, and result in an improvement of the calculation of single neutron scattering quantities. In this work, we discuss the importance of taking into account self-diffusion in liquids to accurately describe the neutron scattering at low neutron energies (quasi-elastic peak problem. To improve modeling of heavy water, it is important to take into account temperature-dependent static structure factors and apply Sköld approximation to the coherent inelastic components of the scattering matrix. The usage of the new set of scattering matrices and cross-sections improves the calculation of thermal critical systems moderated and/or reflected with light/heavy water obtained from the International Criticality Safety Benchmark Evaluation Project (ICSBEP handbook. For example, the use of the new thermal scattering library for heavy water, combined with the ROSFOND-2010 evaluation of the cross sections for deuterium, results in an improvement of the C/E ratio in 48 out of

  3. New evaluation of thermal neutron scattering libraries for light and heavy water

    Science.gov (United States)

    Marquez Damian, Jose Ignacio; Granada, Jose Rolando; Cantargi, Florencia; Roubtsov, Danila

    2017-09-01

    In order to improve the design and safety of thermal nuclear reactors and for verification of criticality safety conditions on systems with significant amount of fissile materials and water, it is necessary to perform high-precision neutron transport calculations and estimate uncertainties of the results. These calculations are based on neutron interaction data distributed in evaluated nuclear data libraries. To improve the evaluations of thermal scattering sub-libraries, we developed a set of thermal neutron scattering cross sections (scattering kernels) for hydrogen bound in light water, and deuterium and oxygen bound in heavy water, in the ENDF-6 format from room temperature up to the critical temperatures of molecular liquids. The new evaluations were generated and processable with NJOY99 and also with NJOY-2012 with minor modifications (updates), and with the new version of NJOY-2016. The new TSL libraries are based on molecular dynamics simulations with GROMACS and recent experimental data, and result in an improvement of the calculation of single neutron scattering quantities. In this work, we discuss the importance of taking into account self-diffusion in liquids to accurately describe the neutron scattering at low neutron energies (quasi-elastic peak problem). To improve modeling of heavy water, it is important to take into account temperature-dependent static structure factors and apply Sköld approximation to the coherent inelastic components of the scattering matrix. The usage of the new set of scattering matrices and cross-sections improves the calculation of thermal critical systems moderated and/or reflected with light/heavy water obtained from the International Criticality Safety Benchmark Evaluation Project (ICSBEP) handbook. For example, the use of the new thermal scattering library for heavy water, combined with the ROSFOND-2010 evaluation of the cross sections for deuterium, results in an improvement of the C/E ratio in 48 out of 65

  4. Neutron scattering from adsorbed species

    International Nuclear Information System (INIS)

    Shuwang An

    1998-01-01

    Neutron reflection has been used to investigate the structure of layers of water-soluble diblock copolymers poly(2-(dimethylamino)ethyl methacrylate-block-methyl methacrylate (poly(DMAEMA-b-MMA)) (70 mol% DMAEMA, M n = 10k, 80 mol% DMAEMA, M n = 10k, and 70 mol% DMAEMA, M n = 20k) adsorbed at the air-liquid and solid-liquid interfaces. The surface tension behaviour of these copolymers at the air-liquid interface has also been investigated. The study of the structure of layers of poly(DMAEMA-b-MMA) adsorbed at the air-water interface forms the main part of the thesis. The surface structure, the effects of pH and ionic strength, and the effects of composition and molecular weight of the copolymers have been studied systematically. For the 70%-10k copolymer at pH 7.5, the adsorption isotherm shows that there is a surface phase transition. The concentration of copolymer at which the phase transition occurs is close to that at which micellar aggregation in the bulk solution also occurs. At low concentrations (below the CMC), the two blocks of the copolymer are approximately uniformly distributed in the direction normal to the interface and the layer is partially immersed in water. At high concentrations (above the CMC), the adsorbed layer has a cross-sectional structure resembling that expected for a micelle with the majority of the MMA blocks forming the core. The outer layers, comprising predominantly DMAEMA blocks, are not equivalent, being more highly extended on the aqueous side of the interface. The effects of pH and added electrolyte on the structure of layers of the 70%-10k copolymer show that the layered structure is promoted by any changes in the bulk solution that enhance the surface coverage but is inhibited by an increase in the fractional charge on the polyelectrolyte part of the copolymer. The effect of lowering the pH is to increase the positive charge on the weak polyelectrolyte block. Addition of electrolyte generally enhances the amount adsorbed and

  5. Density-dependent Hartree-Fock response functions in quasi-elastic electron scattering on 12C and related sum rules

    International Nuclear Information System (INIS)

    Kohno, M.

    1983-01-01

    We report fully consistent calculations of the longitudinal and transverse response functions of the inclusive quasi-elastic electron scattering on 12 C in the Hartree-Fock approximation. The distorted wave for the outgoing nucleon is constructed from the same non-local Hartree-Fock field as in the ground-state description. Thus the orthogonality and Pauli principle requirements are naturally satisfied. The theoretical prediction, based on the standard density-dependent effective interaction (GO force), shows a good correspondence to the experimental data. Since the calculated response functions automatically satisfy the relevant sum rule, this work illuminates the well-known puzzle concerning the longitudinal part, which remains to be solved. We study the energy-weighted sum rules and discuss effects beyond the mean-field approximation. Meson-exchange-current contributions to the transverse response function are also estimated and found to be small due to cancellations among them. (orig.)

  6. Neutron scattering on equilibrium and nonequilibrium phonons, excitons and polaritons

    International Nuclear Information System (INIS)

    Broude, V.L.; Sheka, E.F.

    1978-01-01

    A number of problems of solid-state physics representing interest for neutron spectroscopy of future is considered. The development of the neutron inelastic scattering spectroscopy (neutron spectroscopy of equilibrium phonons) is discussed with application to nuclear dynamics of crystals in the thermodynamic equilibrium. The results of high-flux neutron source experiments on molecular crystals are presented. The advantages of neutron inelastic scattering over optical spectroscopy are discussed. The spectroscopy of quasi-equilibrium and non-equilibrium quasi-particles is discussed. In particular, the neutron scattering on polaritons, excitons in thermal equilibrium and production of light-excitons are considered. The problem of the possibility of such experiments is elucidated

  7. Polarized neutron inelastic scattering experiments on spin dynamics

    International Nuclear Information System (INIS)

    Kakurai, Kazuhisa

    2016-01-01

    The principles of polarized neutron scattering are introduced and examples of polarized neutron inelastic scattering experiments on spin dynamics investigation are presented. These examples should demonstrate the importance of the polarized neutron utilization for the investigation of non-trivial magnetic ground and excited states in frustrated and low dimensional quantum spin systems. (author)

  8. Neutron-scattering studies of chromatin

    International Nuclear Information System (INIS)

    Bradbury, E.M.; Baldwin, J.P.; Carpenter, B.G.; Hjelm, R.P.; Hancock, R.; Ibel, K.

    1976-01-01

    It is clear that a knowledge of the basic molecular structure of chromatin is a prerequisite for any progress toward an understanding of chromosome organization. With a two-component system, protein and nucleic acid, neutrons have a particularly powerful application to studies of the spatial arrangements of these components because of the ability, by contrast matching with H 2 O-D 2 O mixtures, to obtain neutron-scattering data on the individual components. With this approach it has been shown that the neutron diffraction of chromatin is consistent with a ''beads on a string'' model in which the bead consists of a protein core with DNA coiled on the outside. However, because chromatin is a gel and gives limited structural data, confirmation of such a model requires extension of the neutron studies by deuteration of specific chromatin components and the isolation of chromatin subunits. Although these studies are not complete, the neutron results so far obtained support the subunit model described above

  9. Scattering of neutrons and critical phenomena in antiferromagnetic fermi liquid

    International Nuclear Information System (INIS)

    Akhiezer, I.A.; Barannik, E.A.

    1980-01-01

    The scattering of slow neutrons in an antiferromagnetic with collectivized magnetic electrons is considered and it is shown to significantly differ from the neutron scattering in an antiferromagnetic with localized magnetic electrons. The behaviour of scattering cross sections and fluctuation correlators near the Neel point is studied. These magnitudes are shown to increase with the critical index r=-1 [ru

  10. Quantum effects in deep inelastic neutron scattering

    International Nuclear Information System (INIS)

    Mayers, J.

    1989-07-01

    In the Impulse Approximation (IA), which is used to interpret deep inelastic neutron scattering (DINS) measurements, it is assumed both that the target system can be treated as a gas of free atoms and that the struck atom recoils freely after the collision with the neutron. Departures from the IA are generally attributed to final state effects (FSE), which are due to the inaccuracy of the latter assumption. However it is shown that even when FSE are neglected, significant departures from the IA occur at low temperatures due to inaccuracies in the former assumption. These are referred to as initial state effects (ISE) and are due to the quantum nature of the initial state. Comparison with experimental data and exactly soluble models shows that ISE largely account for observed asymmetries and peak shifts in the neutron scattering function S(q,ω), compared with the IA prediction. It is shown that when FSE are neglected, ISE can also be neglected when either the momentum transfer or the temperature is high. Finally it is shown that FSE should be negligible at high momentum transfers in systems other than quantum fluids and that therefore in this regime the IA is reached in such systems. (author)

  11. Probing fine magnetic particles with neutron scattering

    International Nuclear Information System (INIS)

    Pynn, R.

    1991-01-01

    Because thermal neutrons are scattered both by nuclei and by unpaired electrons, they provide an ideal probe for studying the atomic and magnetic structures of fine-grained magnetic materials, including nanocrystalline solids, thin epitaxial layers, and colloidal suspensions of magnetic particles, known as ferrofluids. Diffraction, surface reflection, and small angle neutron scattering (SANS) are the techniques used. With the exception of surface reflection, these methods are described in this article. The combination of SANS with refractive-index matching and neutron polarisation analysis is particularly powerful because it allows the magnetic and atomic structures to be determined independently. This technique has been used to study both dilute and concentrated ferrofluid suspensions of relatively monodisperse cobalt particles, subjected to a series of applied magnetic fields. The size of the cobalt particle core and the surrounding surfactant layer were determined. The measured interparticle structure factor agrees well with a recent theory that allows correlations in binary mixtures of magnetic particles to be calculated in the case of complete magnetic alignment. When one of the species in such a binary mixture is a nonmagnetic, cyclindrical macromolecule, application of a magnetic field leads to some degree of alignment of the nonmagnetic species. This result has been demonstrated with tobacco mosaic virus suspended in a water-based ferrofluid

  12. Neutron Scattering Differential Cross Sections for 12C

    Science.gov (United States)

    Byrd, Stephen T.; Hicks, S. F.; Nickel, M. T.; Block, S. G.; Peters, E. E.; Ramirez, A. P. D.; Mukhopadhyay, S.; McEllistrem, M. T.; Yates, S. W.; Vanhoy, J. R.

    2016-09-01

    Because of the prevalence of its use in the nuclear energy industry and for our overall understanding of the interactions of neutrons with matter, accurately determining the effects of fast neutrons scattering from 12C is important. Previously measured 12C inelastic neutron scattering differential cross sections found in the National Nuclear Data Center (NNDC) show significant discrepancies (>30%). Seeking to resolve these discrepancies, neutron inelastic and elastic scattering differential cross sections for 12C were measured at the University of Kentucky Acceleratory Laboratory for incident neutron energies of 5.58, 5.83, and 6.04 MeV. Quasi mono-energetic neutrons were scattered off an enriched 12C target (>99.99%) and detected by a C6D6 liquid scintillation detector. Time-of-flight (TOF) techniques were used to determine scattered neutron energies and allowed for elastic/inelastic scattering distinction. Relative detector efficiencies were determined through direct measurements of neutrons produced by the 2H(d,n) and 3H(p,n) source reactions, and absolute normalization factors were found by comparing 1H scattering measurements to accepted NNDC values. This experimental procedure has been successfully used for prior neutron scattering measurements and seems well-suited to our current objective. Significant challenges were encountered, however, with measuring the neutron detector efficiency over the broad incident neutron energy range required for these measurements. Funding for this research was provided by the National Nuclear Security Administration (NNSA).

  13. Polarized neutron scattering on HYSPEC: the HYbrid SPECtrometer at SNS

    Energy Technology Data Exchange (ETDEWEB)

    Zaliznyak, Igor [Brookhaven National Laboratory (BNL); Savici, Andrei T [ORNL; Garlea, Vasile O [ORNL; Winn, Barry L [ORNL; Schneelock, John [Brookhaven National Laboratory (BNL); Tranquada, John M. [Brookhaven National Laboratory (BNL); Gu, G. D. [Brookhaven National Laboratory (BNL); Wang, Aifeng [Brookhaven National Laboratory (BNL); Petrovic, C [Brookhaven National Laboratory (BNL)

    2017-01-01

    We describe some of the first polarized neutron scattering measurements performed at HYSPEC spectrometer at the Spallation Neutron Source, Oak Ridge National Laboratory. We discuss details of the instrument setup and the experimental procedures in the mode with the full polarization analysis. Examples of the polarized neutron diffraction and the polarized inelastic neutron data obtained on single crystal samples are presented.

  14. Scatterings and reactions by means of polarized neutron beam

    International Nuclear Information System (INIS)

    Koori, N.

    1989-01-01

    A high resolution polarized neutron beam should be prepared for nuclear physics, which will be planned with the new ring cyclotron at RCNP. Studies on scatterings and reactions by means of polarized neutron beams are reviewed briefly. Beam lines for polarized neutrons are summarized. An example of high resolution measurements of neutron induced reactions is described. (author)

  15. Polarized neutron scattering on HYSPEC: the HYbrid SPECtrometer at SNS

    OpenAIRE

    Zaliznyak, Igor A; Savici, Andrei T.; Garlea, V. Ovidiu; Winn, Barry; Filges, Uwe; Schneeloch, John; Tranquada, John M.; Gu, Genda; Wang, Aifeng; Petrovic, Cedomir

    2016-01-01

    We describe some of the first polarized neutron scattering measurements performed at HYSPEC spectrometer at the Spallation Neutron Source, Oak Ridge National Laboratory. We discuss details of the instrument setup and the experimental procedures in the mode with full polarization analysis. Examples of polarized neutron diffraction and polarized inelastic neutron data obtained on single crystal samples are presented.

  16. Annual report on neutron scattering studies in JAERI

    International Nuclear Information System (INIS)

    Sato, Masatoshi; Nishi, Masakazu; Fujishita, Hideshi; Iizumi, Masashi

    1982-07-01

    Neutron scattering studies carried out from September 1979 to August 1981 by Division of Physics, JAERI, and universities with JRR-2 and -3 neutron beam facilities are described: 61 summary reports, and a list of publications. (author)

  17. Study of scattering in bi-dimensional neutron radiographic images

    International Nuclear Information System (INIS)

    Oliveira, K.A.M. de; Crispim, V.R.; Silva, F.C.

    2009-01-01

    The effect of neutron scattering frequently causes distortions in neutron radiographic images and, thus, reduces the quality. In this project, a type of filter, comprised of cadmium (a neutron absorber), was used in the form of a grid to correct this effect. This device generated image data in the discrete shadow bands of the absorber, components relative to neutron scattering on the test object and surroundings. Scattering image data processing, together with the original neutron radiographic image, resulted in a corrected image with improved edge delineation and, thus, greater definition in the neutron radiographic image of the test object. The objective of this study is to propose a theoretical/experimental methodology that is capable of eliminating the components relative to neutron scattering in neutron radiographic images, coming from the material that composes the test object and the materials that compose the surrounding area. (author)

  18. Neutron scattering instrumentation for biology at spallation neutron sources

    Energy Technology Data Exchange (ETDEWEB)

    Pynn, R. [Los Alamos National Laboratory, NM (United States)

    1994-12-31

    Conventional wisdom holds that since biological entities are large, they must be studied with cold neutrons, a domain in which reactor sources of neutrons are often supposed to be pre-eminent. In fact, the current generation of pulsed spallation neutron sources, such as LANSCE at Los Alamos and ISIS in the United Kingdom, has demonstrated a capability for small angle scattering (SANS) - a typical cold- neutron application - that was not anticipated five years ago. Although no one has yet built a Laue diffractometer at a pulsed spallation source, calculations show that such an instrument would provide an exceptional capability for protein crystallography at one of the existing high-power spoliation sources. Even more exciting is the prospect of installing such spectrometers either at a next-generation, short-pulse spallation source or at a long-pulse spallation source. A recent Los Alamos study has shown that a one-megawatt, short-pulse source, which is an order of magnitude more powerful than LANSCE, could be built with today`s technology. In Europe, a preconceptual design study for a five-megawatt source is under way. Although such short-pulse sources are likely to be the wave of the future, they may not be necessary for some applications - such as Laue diffraction - which can be performed very well at a long-pulse spoliation source. Recently, it has been argued by Mezei that a facility that combines a short-pulse spallation source similar to LANSCE, with a one-megawatt, long-pulse spallation source would provide a cost-effective solution to the global shortage of neutrons for research. The basis for this assertion as well as the performance of some existing neutron spectrometers at short-pulse sources will be examined in this presentation.

  19. Neutron scattering studies of the actinides

    International Nuclear Information System (INIS)

    Lander, G.H.

    1979-01-01

    The electronic structure of actinide materials presents a unique example of the interplay between localized and band electrons. Together with a variety of other techniques, especially magnetization and the Mossbauer effect, neutron studies have helped us to understand the systematics of many actinide compounds that order magnetically. A direct consequence of the localization of 5f electrons is the spin-orbit coupling and subsequent spin-lattice interaction that often leads to strongly anisotropic behavior. The unusual phase transition in UO 2 , for example, arises from interactions between quadrupole moments. On the other hand, in the monopnictides and monochalcogenides, the anisotropy is more difficult to understand, but probably involves an interaction between actinide and anion wave functions. A variety of neutron experiments, including form-factor studies, critical scattering and measurements of the elementary excitations have now been performed, and the conceptual picture emerging from these studies will be discussed

  20. Small-angle neutron scattering technique in liquid crystal studies

    International Nuclear Information System (INIS)

    Shahidan Radiman

    2005-01-01

    The following topics discussed: general principles of SAS (Small-angle Neutron Scattering), liquid crystals, nanoparticle templating on liquid crystals, examples of SAS results, prospects of this studies

  1. Significance of collective motions in biopolymers and neutron scattering

    Energy Technology Data Exchange (ETDEWEB)

    Go, Nobuhiro [Kyoto Univ. (Japan)

    1996-05-01

    Importance of collective variable description of conformational dynamics of biopolymers and the vital role that neutron inelastic scattering phenomena would play in its experimental determination are discussed. (author)

  2. Dynamic properties of electrons in solids by neutron scattering

    International Nuclear Information System (INIS)

    Lovesey, S.W.

    1980-12-01

    Illustrative cases of the use of neutron scattering in the study of the electronic properties of materials discussed here include scattering by localised electrons, narrow band materials and electron plasmas. (U.K.)

  3. Magnetic scattering of neutrons by atoms

    International Nuclear Information System (INIS)

    Stassis, C.; Deckman, H.W.

    1976-01-01

    The magnetic scattering of neutrons by an atom or ion possessing both a spin and orbital magnetic moment is examined. For an atom in the 1sup(n) electronic configuration the magnetic scattering amplitude is determined by matrix elements of even-order electric and odd-order magnetic multipoles, whose order of multipolarity k is less than or equal to 21 + 1. The calculation of the matrix elements of these multipoles is separated into evaluating radial matrix elements and matrix elements of the Racah tensors Wsup(0,k) and Wsup(1,k') where k is an even integar less than or equal to 21. The calculation of the matrix elements of these tensors is considerably simplified by selection rules based on the groups Sp(41 + 2), R(21 + 1), R(3) and in the case of f-electrons, the special group G 2 . It is shown that, in the case of elastic scattering by an atom or an ion whose state is a single Russell-Saunders state, the magnetic scattering amplitude can be written in the conventional form p(q)qsub(m).sigma. General expressions for the amplitude p(q) as well as the elastic magnetic form factor are obtained. The evaluation of the coherent magnetic scattering amplitude by an atom in a magnetic field is discussed, and the small-q approximation to the elastic magnetic scattering is considered. The formation is illustrated for the important case of d- and f-electrons. The generalization of the formalism to the case of mixed atomic configurations is examined in some detail. (author)

  4. Symmetry effects in neutron scattering from isotopically enriched Se isotopes

    Energy Technology Data Exchange (ETDEWEB)

    Lachkar, J.; Haouat, G.; McEllistrem, M. T.; Patin, Y.; Sigaud, J.; Cocu, F.

    1975-06-01

    Differential cross sections for neutron elastic and inelastic scattering from {sup 76}Se, {sup 78}Se, {sup 80}Se and {sup 82}Se, have been measured at 8-MeV incident neutron energy and from {sup 76}Se and {sup 82}Se at 6- and 10-MeV incident energies. The differences observed in the elastic scattering cross sections are interpretable as the effects of isospin term in the scattering potentials. A full analysis of the elastic scattering data are presented.

  5. Magnetic Dynamics of Fine Particles Studied by Inelastic Neutron Scattering

    DEFF Research Database (Denmark)

    Hansen, Mikkel Fougt; Bødker, Franz; Mørup, Steen

    2000-01-01

    We give an introduction to inelastic neutron scattering and the dynamic scattering function for magnetic nanoparticles. Differences between ferromagnetic and antiferromagnetic nanoparticles are discussed and we give a review of recent results on ferromagnetic Fe nanoparticles and canted antiferro......We give an introduction to inelastic neutron scattering and the dynamic scattering function for magnetic nanoparticles. Differences between ferromagnetic and antiferromagnetic nanoparticles are discussed and we give a review of recent results on ferromagnetic Fe nanoparticles and canted...

  6. Neutron scattering studies on dUTPase complex in the presence of bioprotectant systems

    Energy Technology Data Exchange (ETDEWEB)

    Varga, B. [Institute of Enzymology, Hungarian Academy of Sciences, POB 7, H-1518, Budapest (Hungary); Migliardo, F. [Dipartimento di Fisica, Universita di Messina, P.O. Box 55, I-98166 Messina (Italy); Takacs, E.; Vertessy, B. [Institute of Enzymology, Hungarian Academy of Sciences, POB 7, H-1518, Budapest (Hungary); Magazu, S. [Dipartimento di Fisica, Universita di Messina, P.O. Box 55, I-98166 Messina (Italy)], E-mail: smagazu@unime.it; Mondelli, C. [CNR-INFM OGG and CRS-SOFT, c/o ILL, BP 156, 38042 Grenoble Cedex 9 (France)

    2008-04-18

    The aim of the present work is to investigate the chemical physics mechanisms of protein stabilization by homologous disaccharides (trehalose, maltose and sucrose). On this purpose the structural and dynamical properties of dUTPase-inhibitor candidate and dUTPase-inhibitor candidate/disaccharide mixtures have been investigated by elastic neutron scattering (ENS), quasi-elastic neutron scattering (QENS) and photon correlation spectroscopy (PCS). The decrease in the ENS intensity profiles vs temperature for the disaccharide-water mixtures is less marked in the case of trehalose/water mixture. This indicates that trehalose shows a larger structural resistance to temperature changes and a higher 'rigidity' in comparison with maltose/H{sub 2}O and sucrose/H{sub 2}O mixtures. In addition the protein/hydrated-disaccharide mixtures show a linear dependence between the solvent viscosity and the local mean-square displacement of hydrated dUTpase/disaccharide systems. This result shows that the protein dynamics is coupled with that of the surrounding matrix. Furthermore, QENS results on the binary disaccharide-H{sub 2}O/D{sub 2}O mixtures indicate that the water dynamics is affected by all the disaccharides and particularly by trehalose. Finally, PCS findings indicate that the protein hydrodynamic radius in solution does not change at low disaccharide concentrations, while reveal, at high disaccharide concentration, a breakdown of the Stokes-Einstein law. The experimental findings are discussed and interpreted in the frame of the current theories.

  7. Investigation of benzene and toluene layers on 0001 surface of graphite by means of neutron scattering

    International Nuclear Information System (INIS)

    Monkenbusch, M.

    1981-01-01

    The structures of benzene (C 6 H 6 , C 6 D 6 ) and toluene (C 6 H 5 -CH 3 , C 6 D 5 -CD 3 ) monolayers on the basal planes of graphite have been investigated by neutron diffraction. The dynamics of the benzene layer has been studied by observing the incoherently, inelastically scattered neutrons using the time-of-flight method. The main results are: Above a phase transition temperature Tsub(c)approx.=145 K benzene on the basal planes of graphite forms a quasi 2D-fluid with high compressibility. For toluene a fluid phase exists above 140 K, between 70 K and 140 K it forms an incommensurate layer and below 70 K a 3x3 structure has been observed. The fluid phase of adsorbed benzene shows a broad quasielastic scattering indicating an effective surface diffusion coefficient of 10 -4 cm 2 /s at 200 K. The inelastic spectrum has been compared with an appropriate lattice dynamical model. The comparison with the data reveals, can be considered as a fairly anharmonic 2D-solid with a static external potential due to the substrate. (orig./HK)

  8. Current status and future development of neutron scattering in CIAE

    International Nuclear Information System (INIS)

    Chen, D.F.; Gou, C.; Ye, C.T.; Guo, L.P.; Sun, K.

    2003-01-01

    Currently, the 15 MW Heavy Water Research Reactor (HWRR) at China Institute of Atomic Energy (CIAE) in Beijing is the only neutron source available for neutron scattering experiments in China. A 60 MW tank-in-pool inverse neutron trap-type research reactor, China Advanced Research Reactor (CARR), now is being built at CIAE to meet the increasing demand of neutron scattering research in China. According to design, the maximum unperturbed thermal neutron flux would be expected to be 8x10 14 n/cm 2 .s in the reflector region. Seven out of nine tangential horizontal beam tubes will be dedicated for neutron scattering experiments. A cold source, a hot source and a 30x60 m 2 guide tube hall will also be constructed. In this paper, a brief introduction of HWRR, the existing neutron scattering facilities and research activities at HWRR, CARR, and the facilities to be built at CARR are presented. (author)

  9. Soller collimators for small angle neutron scattering

    International Nuclear Information System (INIS)

    Crawford, R.K.; Epperson, J.E.; Thiyagarajan, P.

    1989-01-01

    The neutron beam transmitted through the soller collimators on the SAD (Small Angle Diffractometer) instrument at IPNS (Intense Pulsed Neutron Source) showed wings about the main beam. These wings were quite weak, but were sufficient to interfere with the low-Q scattering data. General considerations of the theory of reflection from homogeneous absorbing media, combined with the results from a Monte Carlo simulation, suggested that these wings were due to specular reflection of neutrons from the absorbing material on the surfaces of the collimator blades. The simulations showed that roughness of the surface was extremely important, with wing background variations of three orders of magnitude being observed with the range of roughness values used in the simulations. Based on the results of these simulations, new collimators for SAD were produced with a much rougher 10 B-binder surface coating on the blades. These new collimators were determined to be significantly better than the original SAD collimators. This work suggests that any soller collimators designed for use with long wavelengths should be fabricated with such a rough surface coating, in order to eliminate (or at least minimize) the undesirable reflection effects which otherwise seem certain to occur. 4 refs., 6 figs

  10. New developments in neutron scattering for the study of molecular systems: structure and diffusive motions

    International Nuclear Information System (INIS)

    Volino, F.

    1976-01-01

    After a short review of the main concepts concerning the neutron and its interaction with matter, the authors focus their attention on the study of molecular systems by means of neutron scattering. Instead of reviewing the subject yet again, they limit themselves to the new kind of work which can be done now, with the combined help of high flux reactors and novel instruments. As examples, a few experiments performed at the Institut Laue-Langevin in Grenoble are described: a neutron diffraction study of liquid acetonitrile using a powder diffractometer installed at the hot source; three high-resolution quasi-elastic studies of molecular motions - in an organic solid, (PAA), an organic liquid (C 3 H 6 ) and a liquid crystal (TBBA) - made by combining measurements with high and ultra-high energy resolution spectrometers installed at the cold source. The concept of elastic incoherent structure factor (EISF) is extensively used for the analysis. Finally some prospects on possible future developments are presented. (orig./HK) [de

  11. The TUNL neutron-neutron scattering length experiment

    International Nuclear Information System (INIS)

    Trotter, D.E.G.; Tornow, W.; Howell, C.R.

    1995-01-01

    Since an accurate value for the neutron-neutron (nn) scattering length a nn is of fundamental interest, its determination should not rely on one source of experimental information only. Besides the π d capture reaction, the nd breakup reaction has been the classical reaction used for determining a nn . However, none of the published values for a nn obtained from kinematically complete nd → n+n+p breakup data are based on a rigorous treatment of the three-nucleon continuum. In addition, the scale uncertainty associated with the existing nd breakup cross-section data in the region of the nn final-state interaction peak is too large to allow for a meaningful reanalysis. Therefore, a new kinematically complete nd breakup experiment is underway at TUNL at an incident neutron energy of 13 MeV. State-of-the-art three-nucleon continuum calculations will be used to analyze the data. In order to investigate the possible influence of three-nucleon force effects, a nn will be determined from data taken at four production angles of the nn pair between 20.5 degrees and 43 degrees (lab)

  12. PREFACE: Structure and dynamics determined by neutron and x-ray scattering Structure and dynamics determined by neutron and x-ray scattering

    Science.gov (United States)

    Müller-Buschbaum, Peter

    2011-06-01

    structure of pyroxene-type MnGeO3 G J Redhammer, A Senyshyn, G Tippelt and G Roth Nanostructured diblock copolymer films with embedded magnetic nanoparticles Xin Xia, Ezzeldin Metwalli, Matthias A Ruderer, Volker Körstgens, Peter Busch, Peter Böni and Peter Müller-Buschbaum Thermal expansion of a La-based bulk metallic glass: insight from in situ high-energy x-ray diffraction J Bednarcik, S Michalik, M Sikorski, C Curfs, X D Wang, J Z Jiang and H Franz The slow short-time motions of phospholipid molecules with a focus on the influence of multiple scattering and fitting artefacts Sebastian Busch and Tobias Unruh Quasi-elastic scattering under short-range order: the linear regime and beyond Michael Leitner and Gero Vogl Structural relaxation as seen by quasielastic neutron scattering on viscous Zr-Ti-Cu-Ni-Be droplets F Yang, T Kordel, D Holland-Moritz, T Unruh and A Meyer In situ observation of cluster formation during nanoparticle solution casting on a colloidal film S V Roth, G Herzog, V Körstgens, A Buffet, M Schwartzkopf, J Perlich, M M Abul Kashem, R Döhrmann, R Gehrke, A Rothkirch, K Stassig, W Wurth, G Benecke, C Li, P Fratzl, M Rawolle and P Müller-Buschbaum Inelastic neutron and x-ray scattering from incommensurate magnetic systems Peter Böni, Bertrand Roessli and Klaudia Hradil Development of magnetic moments in Fe1-xNix-alloys Benjamin Glaubitz, Stefan Buschhorn, Frank Brüssing, Radu Abrudan and Hartmut Zabel Modified mode-coupling theory for the collective dynamics of simple liquids B Schmid and W Schirmacher Inelastic neutron and low-frequency Raman scattering in niobium-phosphate glasses: the role of spatially fluctuating elastic and elasto-optic constants A Schulte, W Schirmacher, B Schmid and T Unruh The effect of heat treatment on the internal structure of nanostructured block copolymer films A Sepe, E T Hoppe, S Jaksch, D Magerl, Q Zhong, J Perlich, D Posselt, D-M Smilgies and C M Papadakis Hydrogen release from sodium alanate observed by time

  13. Non-destructive diagnostics of irradiated materials using neutron scattering from pulsed neutron sources

    Energy Technology Data Exchange (ETDEWEB)

    Korenev, Sergey E-mail: sergey_korenev@steris.com; Sikolenko, Vadim

    2004-10-01

    The advantage of neutron-scattering studies as compared to the standard X-ray technique is the high penetration of neutrons that allow us to study volume effects. The high resolution of instrumentation on the basis neutron scattering allows measurement of the parameters of lattice structure with high precision. We suggest the use of neutron scattering from pulsed neutron sources for analysis of materials irradiated with pulsed high current electron and ion beams. The results of preliminary tests using this method for Ni foils that have been studied by neutron diffraction at the IBR-2 (Pulsed Fast Reactor at Joint Institute for Nuclear Research) are presented.

  14. Non-destructive diagnostics of irradiated materials using neutron scattering from pulsed neutron sources

    Science.gov (United States)

    Korenev, Sergey; Sikolenko, Vadim

    2004-09-01

    The advantage of neutron-scattering studies as compared to the standard X-ray technique is the high penetration of neutrons that allow us to study volume effects. The high resolution of instrumentation on the basis neutron scattering allows measurement of the parameters of lattice structure with high precision. We suggest the use of neutron scattering from pulsed neutron sources for analysis of materials irradiated with pulsed high current electron and ion beams. The results of preliminary tests using this method for Ni foils that have been studied by neutron diffraction at the IBR-2 (Pulsed Fast Reactor at Joint Institute for Nuclear Research) are presented.

  15. Next generation neutron scattering at Neutron Science Center project in JAERI

    International Nuclear Information System (INIS)

    Yamada, Yasusada; Watanabe, Noboru; Niimura, Nobuo; Morii, Yukio; Katano, Susumu; Aizawa, Kazuya; Suzuki, Jun-ichi; Koizumi, Satoshi; Osakabe, Toyotaka.

    1997-01-01

    Japan Atomic Energy Research Institute (JAERI) has promoted neutron scattering researches by means of research reactors in Tokai Research Establishment, and proposes 'Neutron Science Research Center' to develop the future prospect of the Tokai Research Establishment. The scientific fields which will be expected to progress by the neutron scattering experiments carried out at the proposed facility in the Center are surveyed. (author)

  16. Wines: water inelastic neutron scattering experimental study

    International Nuclear Information System (INIS)

    Risch, P.; Ait Abderrahim, H.; D'hondt, P.; Malabu, E.

    1997-01-01

    An intercomparison of calculated fast neutron flux (E > 1 MeV) traverse through a very thick water zone obtained using both S N , (DORT) and Monte-Carlo (TRIPOLI and MCBEND) codes in combination with different cross-sections libraries (based on ENDF/B-III, IV, V and VI), showed small discrepancies either between S N , and Monte-Carlo results or even between S N , or Monte-Carlo results when we consider different cross-sections libraries except for S N , calculation when using P 0 , cross-sections. In order to validate our calculations we looked for experimental data. Unfortunately no experiment, dedicated for the fast neutron transport in large thickness of water, was found in the literature. Therefore SCK-CEN and EDF decided to launch the WINES experiment which is dedicated to study this phenomenon. WINES sands for Water Inelastic Neutron scattering Experimental Study. The aim of this experiment is to provide-experimental data for validation of neutron transport codes and nuclear cross-sections libraries used for LWR surveillance dosimetry analysis. The experimental device is made of 1 m 3 cubic plexiglass container filled with demineralized water. At one face of this cube, a 235 U neutron fission source system is screwed. The source device is made of a 235 U (93 % weight enriched) 18.55 x 16 cm 2 plate cladded with aluminium which is inserted in neutron beam emerging from the graphite gas-cooled BR1 reactor. Fission chambers ( 238 U(n,f), 232 Th(n,f), 237 Np(n,f) and 235 U(n,f)) are used to measure the flux traverses on the central axis of the water cube perpendicular to the fission sources. In this paper we will compare the experimental data to the calculated results using the S N , transport code DORT with the P 3 , ELXSIR library, based on ENDF/B-V, and the P 7 -BUGLE-93 library, based on ENDF/B-VI as well as the Monte-Carlo transport code TRIPOLI with a cross-section library based on ENDF/B IV and ENDF/B-VI. (authors)

  17. Inelastic neutron scattering and lattice dynamics of minerals

    Indian Academy of Sciences (India)

    We review current research on minerals using inelastic neutron scattering and lattice dynamics calculations. Inelastic neutron scattering studies in combination with first principles and atomistic calculations provide a detailed understanding of the phonon dispersion relations, density of states and their manifestations in ...

  18. Inelastic neutron scattering and lattice dynamics of minerals

    Indian Academy of Sciences (India)

    Abstract. We review current research on minerals using inelastic neutron scattering and lattice dynamics calculations. Inelastic neutron scattering studies in combination with first principles and atomistic calculations provide a detailed understanding of the phonon dispersion relations, density of states and their ...

  19. Ten year's activity in the field of neutron scattering workshop

    International Nuclear Information System (INIS)

    Hamaguchi, Yoshikazu

    2003-01-01

    'Neutron scattering' is in the frame of the 'Utilization of Research Reactor's of the FNCA (Forum for Nuclear Cooperation in Asia) project, which held the workshops from FY 1992. This report is a summary of the results and activities of neutron scattering workshops and sub-workshops since the start in FY 1992. (author)

  20. Progress in small angle neutron scattering activities in Malaysia

    Energy Technology Data Exchange (ETDEWEB)

    Mohamed, Abudl Aziz Bin [Industrial Technology Division, Malaysian Institute for Nuclear Technology Research (MINT) (Indonesia)

    2000-10-01

    Research activities by use of small angle neutron scattering in Malaysia are briefly reported. Scattered neutron data are displayed in two or three-dimensional isometric view by the data acquisition system. Visual Basic is utilized for data acquisition and MathCad for data processing and analyses. (Y. Kazumata)

  1. Progress in small angle neutron scattering activities in Malaysia

    International Nuclear Information System (INIS)

    Mohamed, Abudl Aziz Bin

    2000-01-01

    Research activities by use of small angle neutron scattering in Malaysia are briefly reported. Scattered neutron data are displayed in two or three-dimensional isometric view by the data acquisition system. Visual Basic is utilized for data acquisition and MathCad for data processing and analyses. (Y. Kazumata)

  2. Investigation of the setting reaction in magnesium phosphate ceramics with quasielastic neutron scattering

    Czech Academy of Sciences Publication Activity Database

    Viani, Alberto; Zbiri, M.; Bordallo, H. N.; Gualtieri, A. F.; Mácová, Petra

    2017-01-01

    Roč. 121, č. 21 (2017), s. 11355-11367 ISSN 1932-7447 R&D Projects: GA MŠk(CZ) LO1219 Keywords : magnesium potassium phosphate ceramics * amorphous materials * NMR-spectroscopy Subject RIV: JH - Ceramics, Fire-Resistant Materials and Glass OBOR OECD: Ceramics Impact factor: 4.536, year: 2016 http://pubs.acs.org/doi/abs/10.1021/acs.jpcc.7b01396

  3. Quasielastic reactions

    International Nuclear Information System (INIS)

    Hansen, O.

    1983-01-01

    A brief review is presented of the experimental and theoretical situation regarding transfer reactions and inelastic scattering. In the first category there is little (very little) precision data for heavy projectiles and consequently almost no experience with quantitative theoretical analysis. For the inelastic scattering the rather extensive data strongly supports the coupled channels models with collective formfactors. At the most back angles, at intensities about 10 -5 of Rutherford scattering, a second, compound-like mechanism becomes dominant. The description of the interplay of these two opposite mechanisms provides a new challenge for our understanding

  4. Fast diffusion in the intermetallics Ni3Sb and Fe3Si: a neutron scattering study

    International Nuclear Information System (INIS)

    Randl, O.G.

    1994-02-01

    We present the results of neutron scattering experiments designed to elucidate the reason for the extraordinarily fast majority component diffusion in two intermetallic alloys of DO 3 structure, Fe 3 Si and Ni 3 Sb: We have performed diffraction measurements in order to determine the crystal structure and the state of order of both alloys as a function of composition and temperature. The results on Fe 3 Si essentially confirm the classical phase diagram: The alloys of a composition between 16 and 25 at % Si are DO 3 -ordered at room temperature and disorder at high temperatures. The high-temperature phase Ni 3 Sb also crystallizes in the DO 3 structure. Vacancies are created in one Ni sublattice at Sb contents beyond 25 at %. In a second step the diffusion mechanism in Ni 3 Sb has been studied by means of quasielastic neutron scattering. The results are reconcileable with a very simple NN jump model between the two different Ni sublattices. Finally, the lattice dynamics of Fe 3 Si and Ni 3 Sb has been studied by inelastic neutron scattering in dependence of temperature (both alloys) and alloy composition (Fe 3 Si only). The results on Fe 3 Si indicate clearly that phonon enhancement is not the main reason for fast diffusion in this alloy. In Ni 3 Sb no typical signs of phonon-enhanced diffusion have been found either. As a conclusion, fast diffusion in DO 3 intermetallics is explained by extraordinarily high vacancy concentrations (several atomic percent) in the majority component sublattices. (author)

  5. The contribution of neutron scattering to molecular biology

    International Nuclear Information System (INIS)

    Stuhrmann, H.B.

    1983-01-01

    About half of the atoms of living cells are hydrogens, and nearly all biological applications of neutron scattering rely on the well-known difference in the scattering lengths of the proton and the deuteron. This introduces us to a wide variety of biological problems, which are related with hydrogen in water, proteins, nucleic acids and lipids. Neutron scattering gives an answer to both structural and dynamical aspects of the system in question. With deuterium labelled samples unambiguous information about molecular structure and motion becomes accessible. The architecture of viruses, cell membranes and gene expressing molecules has become a lot clearer with neutron scattering. (author)

  6. Neutron scattering studies of the heavy Fermion superconductors

    International Nuclear Information System (INIS)

    Goldman, A.I.

    1985-01-01

    Recent neutron scattering measurements of the heavy Fermion superconductors are described. Those materials offer an exciting opportunity for neutron scattering since the f-electrons, which couple directly to magnetic scattering measurements, seem to be the same electrons which form the superconducting state below T/sub c/. In addition, studies of the magnetic fluctuations in these, and other heavy Fermion systems, by inelastic magnetic neutron scattering can provide information about the nature of the low temperature Fermi liquid character of these novel compounds

  7. Debye-Waller Factor in Neutron Scattering by Ferromagnetic Metals

    Science.gov (United States)

    Paradezhenko, G. V.; Melnikov, N. B.; Reser, B. I.

    2018-04-01

    We obtain an expression for the neutron scattering cross section in the case of an arbitrary interaction of the neutron with the crystal. We give a concise, simple derivation of the Debye-Waller factor as a function of the scattering vector and the temperature. For ferromagnetic metals above the Curie temperature, we estimate the Debye-Waller factor in the range of scattering vectors characteristic of polarized magnetic neutron scattering experiments. In the example of iron, we compare the results of harmonic and anharmonic approximations.

  8. Hydrogen diffusion in the storage compound Ti sub(0.8) Zr sub(0.2)CrMnH3 studied by neutron scattering

    International Nuclear Information System (INIS)

    Pugliesi, R.

    1983-01-01

    The hydrogen diffusion in the storage material Ti sub(0.8) Zr sub(0.2)CrMnH 3 has been studied in the temperature range of 260 to 360K, by means of the quasi-elastic neutron scattering technique. The experimental measurements have been performed using a high resolution backscattering spectrometer. The half widths at half maximum of the quasi-elastic line have been determined for momentum transfers in the range 0.24 to 1.85 A -1 . The data, corrected for multiple scattering effect, have been analysed in term of simple diffusion and jump diffusion models. From the diffusion coefficients determined at different temperatures, the following Arrhenius equation was obtained: D= (3+-1) x 10 -8 m 2 /s exp [-(220+-20 meV/kT] yielding a diffusion coefficient at room temperature of 6.0 x 10 -12 m 2 /s. This comparatively fast hydrogen diffusion is not the rate determining step in the absorption and desorption kinetics. The results at large momentum transfers show evidence for the existence of more than one component in the quasi-elastic spectra. This fact has been explained considering the diffusion governed by the existence of energetically different interstitial sites and by blocking effects due to the high hydrogen concentration. (Author) [pt

  9. Optimising polarised neutron scattering measurements--XYZ and polarimetry analysis

    International Nuclear Information System (INIS)

    Cussen, L.D.; Goossens, D.J.

    2002-01-01

    The analytic optimisation of neutron scattering measurements made using XYZ polarisation analysis and neutron polarimetry techniques is discussed. Expressions for the 'quality factor' and the optimum division of counting time for the XYZ technique are presented. For neutron polarimetry the optimisation is identified as analogous to that for measuring the flipping ratio and reference is made to the results already in the literature

  10. Optimising polarised neutron scattering measurements--XYZ and polarimetry analysis

    CERN Document Server

    Cussen, L D

    2002-01-01

    The analytic optimisation of neutron scattering measurements made using XYZ polarisation analysis and neutron polarimetry techniques is discussed. Expressions for the 'quality factor' and the optimum division of counting time for the XYZ technique are presented. For neutron polarimetry the optimisation is identified as analogous to that for measuring the flipping ratio and reference is made to the results already in the literature.

  11. Slow neutron scattering by water molecules

    Energy Technology Data Exchange (ETDEWEB)

    Stancic, V [Boris Kidric Institute of Nuclear Sciences Vinca, Beograd (Yugoslavia)

    1970-07-01

    In this work some new, preliminary formulae for slow neutron scattering cross section calculation by heavy and light water molecules have been done. The idea was to find, from the sum which exists in well known Nelkin model, other cross sections in a more simple analytical form, so that next approximations may be possible. In order to sum a series it was starting from Euler-Mclaurin formula. Some new summation formulae have been derived there, and defined in two theorems. Extensive calculations, especially during the evaluation of residues, have been made at the CDC 3600 computer. validation of derived formulae was done by comparison with the BNL-325 results. Good agreement is shown. (author)

  12. Lattice Waves, Spin Waves, and Neutron Scattering

    Science.gov (United States)

    Brockhouse, Bertram N.

    1962-03-01

    Use of neutron inelastic scattering to study the forces between atoms in solids is treated. One-phonon processes and lattice vibrations are discussed, and experiments that verified the existence of the quantum of lattice vibrations, the phonon, are reviewed. Dispersion curves, phonon frequencies and absorption, and models for dispersion calculations are discussed. Experiments on the crystal dynamics of metals are examined. Dispersion curves are presented and analyzed; theory of lattice dynamics is considered; effects of Fermi surfaces on dispersion curves; electron-phonon interactions, electronic structure influence on lattice vibrations, and phonon lifetimes are explored. The dispersion relation of spin waves in crystals and experiments in which dispersion curves for spin waves in Co-Fe alloy and magnons in magnetite were obtained and the reality of the magnon was demonstrated are discussed. (D.C.W)

  13. Neutron scattering applied to environmental waste containment

    International Nuclear Information System (INIS)

    Elcombe, M.M.; Studer, A.J.; Waring, C.L.

    1998-01-01

    Full text: A major environmental problem in Australia occurs at mine sites, where rock dumps and tailings dams are still causing problems many years after the mines have ceased operation. ANSTO has developed a method of producing a neutral barrier in-situ, which reduces water flow through the waste material. This in turn prevents water carrying waste products out into the wider environment. Both the loose grained sand substrate and the Neutral Barrier produced are crystalline and therefore amenable to diffraction techniques. In recent laboratory experiments neutron scattering has been used to confirm the presence of the barrier and measure the amount of calcite forming the barrier, at centimetre depths below the surface. The results of these measurements will be presented

  14. Inelastic Neutron Scattering Study of Mn

    Energy Technology Data Exchange (ETDEWEB)

    Zhong, Y.; Sarachik, M.P.; Friedman, J.R.; Robinson, R.A.; Kelley, T.M.; Nakotte, H.; Christianson, A.C.; Trouw, F.; Aubin, S.M.J.; Hendrickson, D.N.

    1998-11-09

    The authors report zero-field inelastic neutron scattering experiments on a 14-gram deuterated sample of Mn{sub 12}-Acetate consisting of a large number of identical spin-10 magnetic clusters. Their resolution enables them to see a series of peaks corresponding to transitions between the anisotropy levels within the spin-10 manifold. A fit to the spin Hamiltonian H = {minus}DS{sub z}{sup 2} + {mu}{sub B}B{center_dot}g{center_dot}S-BS{sub z}{sup 4} + C(S{sub +}{sup 4} + S{sub {minus}}{sup 4}) yields an anisotropy constant D = (0.54 {+-} 0.02) K and a fourth-order diagonal anisotropy coefficient B = (1.2 {+-} 0.1) x 10{sup {minus}3}K. Unlike EPR measurements, their experiments do not require a magnetic field and yield parameters that do not require knowledge of the g-value.

  15. Neutron Compton scattering from selectively deuterated acetanilide

    Science.gov (United States)

    Wanderlingh, U. N.; Fielding, A. L.; Middendorf, H. D.

    With the aim of developing the application of neutron Compton scattering (NCS) to molecular systems of biophysical interest, we are using the Compton spectrometer EVS at ISIS to characterize the momentum distribution of protons in peptide groups. In this contribution we present NCS measurements of the recoil peak (Compton profile) due to the amide proton in otherwise fully deuterated acetanilide (ACN), a widely studied model system for H-bonding and energy transfer in biomolecules. We obtain values for the average width of the potential well of the amide proton and its mean kinetic energy. Deviations from the Gaussian form of the Compton profile, analyzed on the basis of an expansion due to Sears, provide data relating to the Laplacian of the proton potential.

  16. Slow neutron scattering by water molecules

    International Nuclear Information System (INIS)

    Stancic, V.

    1970-01-01

    In this work some new, preliminary formulae for slow neutron scattering cross section calculation by heavy and light water molecules have been done. The idea was to find, from the sum which exists in well known Nelkin model, other cross sections in a more simple analytical form, so that next approximations may be possible. In order to sum a series it was starting from Euler-Mclaurin formula. Some new summation formulae have been derived there, and defined in two theorems. Extensive calculations, especially during the evaluation of residues, have been made at the CDC 3600 computer. validation of derived formulae was done by comparison with the BNL-325 results. Good agreement is shown. (author)

  17. Neutron detection efficiency determinations for the TUNL neutron-neutron and neutron-proton scattering-length measurements

    Energy Technology Data Exchange (ETDEWEB)

    Trotter, D.E. Gonzalez [Department of Physics, Duke University and Triangle Universities Nuclear Laboratory, Durham, NC 27708-0308 (United States)], E-mail: crowell@tunl.duke.edu; Meneses, F. Salinas [Department of Physics, Duke University and Triangle Universities Nuclear Laboratory, Durham, NC 27708-0308 (United States); Tornow, W. [Department of Physics, Duke University and Triangle Universities Nuclear Laboratory, Durham, NC 27708-0308 (United States)], E-mail: tornow@tunl.duke.edu; Crowell, A.S.; Howell, C.R. [Department of Physics, Duke University and Triangle Universities Nuclear Laboratory, Durham, NC 27708-0308 (United States); Schmidt, D. [Physikalisch-Technische Bundesanstalt, D-38116, Braunschweig (Germany); Walter, R.L. [Department of Physics, Duke University and Triangle Universities Nuclear Laboratory, Durham, NC 27708-0308 (United States)

    2009-02-11

    The methods employed and the results obtained from measurements and calculations of the detection efficiency for the neutron detectors used at Triangle Universities Nuclear Laboratory (TUNL) in the simultaneous determination of the {sup 1}S{sub 0} neutron-neutron and neutron-proton scattering lengths a{sub nn} and a{sub np}, respectively, are described. Typical values for the detector efficiency were 0.3. Very good agreement between the different experimental methods and between data and calculation has been obtained in the neutron energy range below E{sub n}=13MeV.

  18. Neutron detection efficiency determinations for the TUNL neutron-neutron and neutron-proton scattering-length measurements

    International Nuclear Information System (INIS)

    Trotter, D.E. Gonzalez; Meneses, F. Salinas; Tornow, W.; Crowell, A.S.; Howell, C.R.; Schmidt, D.; Walter, R.L.

    2009-01-01

    The methods employed and the results obtained from measurements and calculations of the detection efficiency for the neutron detectors used at Triangle Universities Nuclear Laboratory (TUNL) in the simultaneous determination of the 1 S 0 neutron-neutron and neutron-proton scattering lengths a nn and a np , respectively, are described. Typical values for the detector efficiency were 0.3. Very good agreement between the different experimental methods and between data and calculation has been obtained in the neutron energy range below E n =13MeV.

  19. Neutron scattering for the analysis of biological structures. Brookhaven symposia in biology. Number 27

    Energy Technology Data Exchange (ETDEWEB)

    Schoenborn, B P [ed.

    1976-01-01

    Sessions were included on neutron scattering and biological structure analysis, protein crystallography, neutron scattering from oriented systems, solution scattering, preparation of deuterated specimens, inelastic scattering, data analysis, experimental techniques, and instrumentation. Separate entries were made for the individual papers.

  20. Magnetic field effects on the soft mode in a singlet ground-state dimer system: a neutron scattering study of Cs3Cr2Br9

    DEFF Research Database (Denmark)

    Leuenberger, Bruno; Gudel, Hans U.; Feile, Rudolf

    1985-01-01

    Neutron scattering experiments in a magnetic field have been performed on the singlet ground-state dimer system Cs3Cr2Br9. At low fields the Zeeman splitting of the soft mode evolves in agreement with the isotropic random-phase approximation (RPA) model, with the notable absence of a quasielastic...... peak. At a temperature of 1.7K the expected long-range magnetic order is not found at the predicted field of 2.8 T, indicating the shortcomings of the isotropic RPA model in the critical region. Magnetic intensity on the weak nuclear Bragg peak (1¯1¯4) indicates a probable ordering with a ferromagnetic...

  1. Introduction to the theory of thermal neutron scattering

    CERN Document Server

    Squires, G L

    2012-01-01

    Since the advent of the nuclear reactor, thermal neutron scattering has proved a valuable tool for studying many properties of solids and liquids, and research workers are active in the field at reactor centres and universities throughout the world. This classic text provides the basic quantum theory of thermal neutron scattering and applies the concepts to scattering by crystals, liquids and magnetic systems. Other topics discussed are the relation of the scattering to correlation functions in the scattering system, the dynamical theory of scattering and polarisation analysis. No previous knowledge of the theory of thermal neutron scattering is assumed, but basic knowledge of quantum mechanics and solid state physics is required. The book is intended for experimenters rather than theoreticians, and the discussion is kept as informal as possible. A number of examples, with worked solutions, are included as an aid to the understanding of the text.

  2. Neutron scattering investigations of frustated magnets

    Science.gov (United States)

    Fennell, Tom

    This thesis describes the experimental investigation of frustrated magnetic systems based on the pyrochlore lattice of corner-sharing tetrahedra. Ho2Ti207 and Dy2Ti207 are examples of spin ices, in which the manifold of disordered magnetic groundstates maps onto that of the proton positions in ice. Using single crystal neutron scattering to measure Bragg and diffuse scattering, the effect of applying magnetic fields along different directions in the crystal was investigated. Different schemes of degeneracy removal were observed for different directions. Long and short range order, and the coexistence of both could be observed by this technique.The field and temperature dependence of magnetic ordering was studied in Ho2Ti207 and Dy2Ti207. Ho2Ti2()7 has been more extensively investigated. The field was applied on [00l], [hh0], [hhh] and [hh2h]. Dy2Ti207 was studied with the field applied on [00l] and [hho] but more detailed information about the evolution of the scattering pattern across a large area of reciprocal space was obtained.With the field applied on [00l] both materials showed complete degeneracy removal. A long range ordered structure was formed. Any magnetic diffuse scattering vanished and was entirely replaced by strong magnetic Bragg scattering. At T =0.05 K both materials show unusual magnetization curves, with a prominent step and hysteresis. This was attributed to the extremely slow dynamics of spin ice materials at this temperature.Both materials were studied in greatest detail with the field applied on [hh0]. The coexistence of long and short range order was observed when the field was raised at T = 0.05 K. The application of a field in this direction separated the spin system into two populations. One could be ordered by the field, and one remained disordered. However, via spin-spin interactions, the field restricted the degeneracy of the disordered spin population. The neutron scattering pattern of Dy2Ti207 shows that the spin system was separated

  3. Multiple small-angle neutron scattering studies of anisotropic materials

    CERN Document Server

    Allen, A J; Long, G G; Ilavsky, J

    2002-01-01

    Building on previous work that considered spherical scatterers and randomly oriented spheroidal scatterers, we describe a multiple small-angle neutron scattering (MSANS) analysis for nonrandomly oriented spheroids. We illustrate this with studies of the multi-component void morphologies found in plasma-spray thermal barrier coatings. (orig.)

  4. Dynamics of liquid N2 studied by neutron inelastic scattering

    DEFF Research Database (Denmark)

    Pedersen, Karen Schou; Carneiro, Kim; Hansen, Flemming Yssing

    1982-01-01

    Neutron inelastic-scattering data from liquid N2 at wave-vector transfer κ between 0.18 and 2.1 Å-1 and temperatures ranging from T=65-77 K are presented. The data are corrected for the contribution from multiple scattering and incoherent scattering. The resulting dynamic structure factor S (κ,ω)...

  5. Adsorption and desorption behaviors of cationic liposome-DNA complexes upon lipofection in inside and outside biomembrane models using a dynamic quasi-elastic laser scattering method.

    Science.gov (United States)

    Uchiyama, Yoshiko; Yui, Hiroharu; Sawada, Tsuguo

    2004-11-01

    The dynamic behaviors of cationic liposome-DNA complexes in inside and outside biomembrane models upon lipofection were investigated using the time-resolved quasi-elastic laser scattering (QELS) method. Inside and outside biomembrane models with similar phospholipid compositions to those in living cells were formed at a tetradecane/phosphate buffered saline (TD/PBS) interface. Cationic liposome-DNA complexes were injected into the buffer subphase, and their adsorption/desorption behaviors at the biomembrane models were monitored through changes in the interfacial tension. We found that the adsorption rate of the complexes increased 2.6 times more in the outside model than in the inside one. The adsorption rate of DNA alone did not show a remarkable difference from one side to the other; however, the adsorption rate of the cationic liposome alone showed a similar tendency to that of the liposome-DNA complex. These results indicated that the difference in lipid composition induced a different dynamic behavior of exogenous biomolecules and that the cationic liposomes played an important role in the faster incorporation of DNA into cells upon lipofection.

  6. Calculation of the RPA response function of nuclei to quasi-elastic electron scattering with a density-dependent NN interaction

    International Nuclear Information System (INIS)

    Caillon, J-C.; Labarsouque, J.

    1997-01-01

    So far, the non-relativistic longitudinal and transverse functions in electron quasi-elastic scattering on the nuclei failed in reproducing satisfactorily the existent experimental data. The calculations including relativistic RPA correlations utilize until now the relativistic Hartree approximation to describe the nuclear matter. But, this provides an incompressibility module two times higher than its experimental value what is an important drawback for the calculation of realistic relativistic RPA correlations. Hence, we have determined the RPA response functions of nuclei by utilising a description of the relativistic nuclear matter leading to an incompressibility module in agreement with the empirical value. To do that we have utilized an interaction in the relativistic Hartree approximation in which we have determined the coupling constants σ-N and ω-N as a function of the density in order to reproduce the saturation curve obtained by a Dirac-Brueckner calculation. The results which we have obtained show that the longitudinal response function and the Coulomb sum generally overestimated when one utilizes the pure relativistic Hartree approximation, are here in good agreement with the experimental data for several nuclei

  7. DISCUS, Neutron Single to Double Scattering Ratio in Inelastic Scattering Experiment by Monte-Carlo

    International Nuclear Information System (INIS)

    Johnson, M.W.

    1993-01-01

    1 - Description of problem or function: DISCUS calculates the ratio of once-scattered to twice-scattered neutrons detected in an inelastic neutron scattering experiment. DISCUS also calculates the flux of once-scattered neutrons that would have been observed if there were no absorption in the sample and if, once scattered, the neutron would emerge without further re-scattering or absorption. Three types of sample geometry are used: an infinite flat plate, a finite flat plate or a finite length cylinder. (The infinite flat plate is included for comparison with other multiple scattering programs.) The program may be used for any sample for which the scattering law is of the form S(/Q/, omega). 2 - Method of solution: Monte Carlo with importance sampling is used. Neutrons are 'forced' both into useful angular trajectories, and useful energy bins. Biasing of the collision point according to the point of entry of the neutron into the sample is also utilised. The first and second order scattered neutron fluxes are calculated in independent histories. For twice-scattered neutron histories a square distribution in Q-omega space is used to sample the neutron coming from the first scattering event, whilst biasing is used for the second scattering event. (A square distribution is used so as to obtain reasonable inelastic-inelastic statistics.) 3 - Restrictions on the complexity of the problem: Unlimited number of detectors. Max. size of (Q, omega) matrix is 39*149. Max. number of points in momentum space for the scattering cross section is 199

  8. Neutron scattering and the search for mechanisms of superconductivity

    DEFF Research Database (Denmark)

    Aeppli, G.; Bishop, D.J.; Broholm, C.

    1999-01-01

    Neutron scattering is a direct probe of mass and magnetization density in solids. We start with a brief review of experimental strategies for determining the mechanisms of superconductivity and how neutron scattering contributed towards our understanding of conventional superconductors. The remai......Neutron scattering is a direct probe of mass and magnetization density in solids. We start with a brief review of experimental strategies for determining the mechanisms of superconductivity and how neutron scattering contributed towards our understanding of conventional superconductors....... The remainder of the article gives examples of neutron results with impact on the search for the mechanism of superconductivity in more recently discovered, 'exotic', materials, namely the heavy fermion compounds and the layered cuprates, (C) 1999 Elsevier Science B.V. All rights reserved....

  9. Elements of slow-neutron scattering basics, techniques, and applications

    CERN Document Server

    Carpenter, J M

    2015-01-01

    Providing a comprehensive and up-to-date introduction to the theory and applications of slow-neutron scattering, this detailed book equips readers with the fundamental principles of neutron studies, including the background and evolving development of neutron sources, facility design, neutron scattering instrumentation and techniques, and applications in materials phenomena. Drawing on the authors' extensive experience in this field, this text explores the implications of slow-neutron research in greater depth and breadth than ever before in an accessible yet rigorous manner suitable for both students and researchers in the fields of physics, biology, and materials engineering. Through pedagogical examples and in-depth discussion, readers will be able to grasp the full scope of the field of neutron scattering, from theoretical background through to practical, scientific applications.

  10. Dynamically Polarized Sample for Neutron Scattering At the Spallation Neutron Source

    International Nuclear Information System (INIS)

    Pierce, Josh; Zhao, J. K.; Crabb, Don

    2009-01-01

    The recently constructed Spallation Neutron Source at the Oak Ridge National Laboratory is quickly becoming the world's leader in neutron scattering sciences. In addition to the world's most intense pulsed neutron source, we are continuously constructing state of the art neutron scattering instruments as well as sample environments to address today and tomorrow's challenges in materials research. The Dynamically Polarized Sample project at the SNS is aimed at taking maximum advantage of polarized neutron scattering from polarized samples, especially biological samples that are abundant in hydrogen. Polarized neutron scattering will allow us drastically increase the signal to noise ratio in experiments such as neutron protein crystallography. The DPS project is near completion and all key components have been tested. Here we report the current status of the project.

  11. Neutron total scattering cross sections of elemental antimony

    Energy Technology Data Exchange (ETDEWEB)

    Smith, A.B.; Guenther, P.T.; Whalen, J.F.

    1982-11-01

    Neutron total cross sections are measured from 0.8 to 4.5 MeV with broad resolutions. Differential-neutron-elastic-scattering cross sections are measured from 1.5 to 4.0 MeV at intervals of 50 to 200 keV and at scattering angles distributed between 20 and 160 degrees. Lumped-level neutron-inelastic-scattering cross sections are measured over the same angular and energy range. The exPerimental results are discussed in terms of an optical-statistical model and are compared with respective values given in ENDF/B-V.

  12. On the theory of ultracold neutrons scattering by Davydov solitons

    International Nuclear Information System (INIS)

    Brizhik, L.S.

    1984-01-01

    Elastic coherent scattering of ultracold neutrons by Davydov solitons in one-dimensional periodic molecular chains without account of thermal oscillations of chain atoms is studied. It is shown that the expression for the differential cross section of the elastic neutron scattering by Davydov soliton breaks down into two components. One of them corresponds to scattering by a resting soliton, the other is proportional to the soliton velocity and has a sharp maximum in the direction of mirror reflection of neutrons from the chain

  13. Local-field refinement of neutron scattering lengths

    Energy Technology Data Exchange (ETDEWEB)

    Sears, V F

    1985-06-01

    We examine the way in which local field effects in the neutron refractive index affect the values of coherent scattering lengths determined by various kinds of neutron optical measurements. We find that under typical experimental conditions these effects are negligible for interferometry measurements but that they are significant for gravity refractometry measurements, producing changes in the effective scattering length of as much as two or three standard deviations in some cases. Refined values of the scattering length are obtained for the thirteen elements for which data are presently available. The special role of local field effects in neutron transmission is also discussed.

  14. Local-field refinement of neutron scattering lengths

    International Nuclear Information System (INIS)

    Sears, V.F.

    1985-01-01

    We examine the way in which local field effects in the neutron refractive index affect the values of coherent scattering lengths determined by various kinds of neutron optical measurements. We find that under typical experimental conditions these effects are negligible for interferometry measurements but that they are significant for gravity refractometry measurements, producing changes in the effective scattering length of as much as two or three standard deviations in some cases. Refined values of the scattering length are obtained for the thirteen elements for which data are presently available. The special role of local field effects in neutron transmission is also discussed. (orig.)

  15. New statistical model of inelastic fast neutron scattering

    International Nuclear Information System (INIS)

    Stancicj, V.

    1975-07-01

    A new statistical model for treating the fast neutron inelastic scattering has been proposed by using the general expressions of the double differential cross section in impuls approximation. The use of the Fermi-Dirac distribution of nucleons makes it possible to derive an analytical expression of the fast neutron inelastic scattering kernel including the angular momenta coupling. The obtained values of the inelastic fast neutron cross section calculated from the derived expression of the scattering kernel are in a good agreement with the experiments. A main advantage of the derived expressions is in their simplicity for the practical calculations

  16. Neutron total scattering cross sections of elemental antimony

    International Nuclear Information System (INIS)

    Smith, A.B.; Guenther, P.T.; Whalen, J.F.

    1982-11-01

    Neutron total cross sections are measured from 0.8 to 4.5 MeV with broad resolutions. Differential-neutron-elastic-scattering cross sections are measured from 1.5 to 4.0 MeV at intervals of 50 to 200 keV and at scattering angles distributed between 20 and 160 degrees. Lumped-level neutron-inelastic-scattering cross sections are measured over the same angular and energy range. The exPerimental results are discussed in terms of an optical-statistical model and are compared with respective values given in ENDF/B-V

  17. Inelastic magnetic scattering of polarized neutrons by a superconducting ring

    International Nuclear Information System (INIS)

    Agafonov, A. I.

    2011-01-01

    The inelastic scattering of cold neutrons by a ring leads to quantum jumps of a superconducting current which correspond to a decrease in the fluxoid quantum number by one or several units while the change in the ring energy is transferred to the kinetic energy of the scattered neutron. The scattering cross sections of transversely polarized neutrons have been calculated for a thin type-II superconductor ring, the thickness of which is smaller than the field penetration depth but larger than the electron mean free path.

  18. Water dynamics as affected by interaction with biomolecules and change of thermodynamic state: a neutron scattering study

    International Nuclear Information System (INIS)

    Orecchini, A; Paciaroni, A; Petrillo, C; Sebastiani, F; Sacchetti, F; De Francesco, A

    2012-01-01

    The dynamics of water as subtly perturbed by both the interaction with biomolecules and the variation of temperature and pressure has been investigated via neutron scattering spectroscopy. A measurement of inelastic neutron scattering devoted to the study of the coherent THz dynamics of water in a water-rich mixture with DNA (hydration level of 1 g DNA/15 g D 2 O) at room temperature is reported. The DNA hydration water coherent dynamics is characterised by the presence of collective modes, whose dispersion relations are similar to those observed in bulk water. These dispersion relations are well described by the interaction model developed in the case of bulk water, and the existence of a fast sound is experimentally demonstrated. The behaviour of the collective water dynamics was complemented by studying the single-particle dynamics of bulk water along the isotherm T = 298 K in the pressure range 0.1-350 MPa by means of incoherent scattering. This experiment is an attempt to simulate the change of the water molecular arrangement due to the interaction with DNA, by increasing the pressure as the presence of the biomolecule produces an increase in the density. An anomaly is found in the behaviour of the relaxation time derived from the quasi-elastic scattering signal, which can be related to the hypothetical second critical point in water. This anomaly and the transition from slow to fast sound take place in the same Q range, thus suggesting that the two phenomena could be related at some microscopic level.

  19. Application of Van Hove theory to fast neutron inelastic scattering

    International Nuclear Information System (INIS)

    Stanicicj, V.

    1974-11-01

    The Vane Hove general theory of the double differential scattering cross section has been used to derive the particular expressions of the inelastic fast neutrons scattering kernel and scattering cross section. Since the considered energies of incoming neutrons being less than 10 MeV, it enables to use the Fermi gas model of nucleons. In this case it was easy to derive an analytical expression for the time-dependent correlation function of the nucleus. Further, by using an impulse approximation and a short-collision time approach, it was possible to derive the analytical expression of the scattering kernel and scattering cross section for the fast neutron inelastic scattering. The obtained expressions have been used for Fe nucleus. It has been shown a surprising agreement with the experiments. The main advantage of this theory is in its simplicity for some practical calculations and for some theoretical investigations of nuclear processes

  20. LANSCE '90: the Manuel Lujan Jr. Neutron Scattering Center

    International Nuclear Information System (INIS)

    Pynn, Roger

    1991-01-01

    This paper describes progress that has been made at the Manuel Lujan Jr. Neutron Scattering Center (LANSCE) during the past two years. Presently, LANSCE provides a higher peak neutron flux than any other pulsed spallation neutron source. There are seven spectrometers for neutron scattering experiments that are operated for a national user program sponsored by the U.S. Department of Energy. Two more spectrometers are under construction. Plans have been made to raise the number of beam holes available for instrumentation and to improve the efficiency of the target/moderator system. (author)

  1. LANSCE '90: The Manuel Lujan Jr. Neutron Scattering Center

    International Nuclear Information System (INIS)

    Pynn, R.

    1990-01-01

    This paper describes progress that has been made at the Manuel Lujan Jr. Neutron Scattering Center (LANSCE) during the past two years. Presently, LANSCE provides a higher peak neutron flux than any other pulsed spallation neutron source. There are seven spectrometers for neutron scattering experiments that are operated for a national user program sponsored by the US Department of Energy. Two more spectrometers are under construction. Plans have been made to raise the number of beam holes available for instrumentation and to improve the efficiency of the target/moderator system. 9 refs., 4 figs

  2. Early history of neutron scattering at Oak Ridge

    International Nuclear Information System (INIS)

    Wilkinson, M.K.

    1985-07-01

    Most of the early development of neutron scattering techniques utilizing reactor neutrons occurred at the Oak Ridge National Laboratory during the years immediately following World War II. C.G. Shull, E.O. Wollan, and their associates systematically established neutron diffraction as a quantitative research tool and then applied this technique to important problems in nuclear physics, chemical crystallography, and magnetism. This article briefly summarizes the very important research at ORNL during this period, which laid the foundation for the establishment of neutron scattering programs throughout the world. 47 refs., 10 figs

  3. Plane-wave impulse approximation extraction of the neutron magnetic form factor from Quasi-Elastic 3(rvec H)e((rvec e),e(prime)) at Q2 = 0.3 to 0.6 (GeV/c)2

    International Nuclear Information System (INIS)

    Xu, W.; Anderson, B.; Auberbach, L.; Averett, T.; Bertozzi, W.; Black, T.; Calarco, J.; Cardman, L.; Cates, G.D.; Chai, Z.W.; Chen, J.P.; Choi, S.; Chudakov, E.; Churchwell, S.; Corrado, G.S.; Crawford, C.; Dale, D.; Deur, A.; Djawotho, P.; Donnelly, T.W.; Dutta, D.; Finn, J.M.; Gao, H.; Gilman, R.; Glamazdin, A.V.; Glashausser, C.; Gloeckle, Walter; Golak, J.; Gomez, J.; Gorbenko, V.G.; Hansen, J.O.; Hersman, F.W.; Higinbotham, D.W.; Holmes, R.; Howell, C.R.; Hughes, E.; Humensky, B.; Incerti, S.; Jager, C.W. de; Jensen, J.S.; Jiang, X.; Jones, C.E.; Jones, M.; Kahl, R.; Kamada, H.; Kievsky, A.; Kominis, I.; Korsch, W.; Kramer, K.; Kumbartzki, G.; Kuss, M.; Lakuriqi, E.; Liang, M.; Liyanage, N.; LeRose, J.; Malov, S.; Margaziotis, D.J.; Martin, J.W.; McCormick, K.; McKeown, R. D.; McIlhany, K.; Meziani, Z.E.; Michaels, R.; Miller, G.W.; Mitchell, J.; Nanda, S.; Pace, E.; Pavlin, T.; Petratos, G.G.; Pomatsalyuk, R.I.; Pripstein, D.; Prout, D.; Ransome, R.D.; Roblin, Y.; Rvachev, M.; Saha, A.; Salme, G.; Schnee, M.; Shin, T.; Slifer, K.; Souder, P.A.; Strauch, S.; Suleiman, R.; Sutter, M.; Tipton, B.; Todor, L.; Viviani, M.; Vlahovic, B.; Watson, J.; Williamson, C.F.; Witala, H.; Wojtsekhowski, B.; Xiong, F.; Yeh, J.; Zolnierczuk, P.

    2003-01-01

    A high precision measurement of the transverse spin-dependent asymmetry A T in 3 (rvec H)e((rvec e),e(prime)) quasielastic scattering was performed in Hall A at Jefferson Lab at values of the squared four-momentum transfer, Q 2 , between 0.1 and 0.6 (GeV/c) 2 . A T is sensitive to the neutron magnetic form factor, G M n . Values of G M n at Q 2 = 0.1 and 0.2 (GeV/c) 2 , extracted using Faddeev calculations, were reported previously. Here, we report the extraction of G M n for the remaining Q 2 -values in the range from 0.3 to 0.6 (GeV/c) 2 using a Plane-Wave Impulse Approximation calculation. The results are in good agreement with recent precision data from experiments using a deuterium target

  4. Applications of the quasi-elastic light scattering to the study of dynamic properties of charged macro-molecules

    International Nuclear Information System (INIS)

    Gouesin-Menez, Renee

    1979-01-01

    The object of this research thesis is to study the modifications of dynamic properties of a macromolecule under the influence of variations of its medium, by using a frequency analysis of the spectrum of light scattered by a solution of particles. Thus, an important part of this thesis addresses the study and development of the scattering method and of its analysis by 'photon pulses', and the development and adjustment of an electrophoretic device to study light scattering by molecules submitted to an electric field. Then, hydrodynamic characteristics of some macromolecules have been measured with or without electric field. The studied molecular systems have been: calibrated spheres of latex polystyrene, a globular protein (bovine serum albumin), a polysaccharide (under the form of a rigid short stick), a flexible linear polyelectrolyte (polymethacrylate), and two DNA samples

  5. Neutron scattering study of yttrium iron garnet

    Science.gov (United States)

    Shamoto, Shin-ichi; Ito, Takashi U.; Onishi, Hiroaki; Yamauchi, Hiroki; Inamura, Yasuhiro; Matsuura, Masato; Akatsu, Mitsuhiro; Kodama, Katsuaki; Nakao, Akiko; Moyoshi, Taketo; Munakata, Koji; Ohhara, Takashi; Nakamura, Mitsutaka; Ohira-Kawamura, Seiko; Nemoto, Yuichi; Shibata, Kaoru

    2018-02-01

    The nuclear and magnetic structure and full magnon dispersions of yttrium iron garnet Y3Fe5O12 have been studied using neutron scattering. The refined nuclear structure is distorted to a trigonal space group of R 3 ¯ . The highest-energy dispersion extends up to 86 meV. The observed dispersions are reproduced by a simple model with three nearest-neighbor-exchange integrals between 16 a (octahedral) and 24 d (tetrahedral) sites, Ja a, Ja d, and Jd d, which are estimated to be 0.00 ±0.05 , -2.90 ±0.07 , and -0.35 ±0.08 meV, respectively. The lowest-energy dispersion below 14 meV exhibits a quadratic dispersion as expected from ferromagnetic magnons. The imaginary part of q -integrated dynamical spin susceptibility χ″(E ) exhibits a square-root energy dependence at low energies. The magnon density of state is estimated from χ″(E ) obtained on an absolute scale. The value is consistent with the single chirality mode for the magnon branch expected theoretically.

  6. Inelastic neutron scattering of amorphous ice

    International Nuclear Information System (INIS)

    Fukazawa, Hiroshi; Ikeda, Susumu; Suzuki, Yoshiharu

    2001-01-01

    We measured the inelastic neutron scattering from high-density amorphous (HDA) and low-density amorphous (LDA) ice produced by pressurizing and releasing the pressure. We found a clear difference between the intermolecular vibrations in HDA and those in LDA ice: LDA ice has peaks at 22 and 33 meV, which are also seen in the spectrum of lattice vibrations in ice crystal, but the spectrum of HDA ice does not have these peaks. The excitation energy of librational vibrations in HDA ice is 10 meV lower than that in LDA ice. These results imply that HDA ice includes 2- and 5-coordinated hydrogen bonds that are created by breakage of hydrogen bonds and migration of water molecules into the interstitial site, while LDA ice contains mainly 4-coordinated hydrogen bonds and large cavities. Furthermore, we report the dynamical structure factor in the amorphous ice and show that LDA ice is more closely related to the ice crystal structure than to HDA ice. (author)

  7. Small-angle neutron scattering studies of sodium butyl benzene

    Indian Academy of Sciences (India)

    Na-NBBS), in aqueous solutions is investigated by small-angle neutron scattering (SANS). Nearly ellipsoidal aggregates of Na-NBBS at concentrations well above its minimum hydrotrope concentration were detected by SANS. The hydrotrope ...

  8. Spectrum of ferromagnetic transition metal magnetic excitations and neutron scattering

    International Nuclear Information System (INIS)

    Kuzemskij, A.L.

    1979-01-01

    Quantum statistical models of ferromagnetic transition metals as well as methods of their solutions are reviewed. The correspondence of results on solving these models and the data on scattering thermal neutrons in ferromagnetic is discussed

  9. Life at extreme conditions: Neutron scattering studies of biological

    Indian Academy of Sciences (India)

    Extremophile bacteria; molecular adaptation; halophile; water dynamics; protein dynamics. ... Results of neutron scattering measurements on the dynamics of proteins ... The experiments were performed on a halophilic protein, and membrane ...

  10. Analysis of inelastic neutron scattering results on model compounds ...

    Indian Academy of Sciences (India)

    Vibrational spectroscopy; nitrogenous bases; inelastic neutron scattering. PACS No. ... obtain good quality, high resolution results in this region. Here the .... knowledge of the character of each molecular transition as well as the calculated.

  11. 3rd AINSE neutron scattering conference, Lucas Heights -AINSE Theatre

    International Nuclear Information System (INIS)

    1986-01-01

    Abstracts of papers, the conference program and general information is included in the conference handbook. The program is divided into the following sessions: hydrogeneous and biological materials, industrial applications, phase transitions, magnetism, small angle neutron scattering and new developments

  12. Applications of neutron scattering in molecular biological research

    International Nuclear Information System (INIS)

    Nierhaus, K.H.

    1984-01-01

    The study of the molecular structure of biological materials by neutron scattering is described. As example the results of the study of the components of a ribosome of Escherichia coli are presented. (HSI) [de

  13. An empirical formula for scattered neutron components in fast neutron radiography

    International Nuclear Information System (INIS)

    Dou Haifeng; Tang Bin

    2011-01-01

    Scattering neutrons are one of the key factors that may affect the images of fast neutron radiography. In this paper, a mathematical model for scattered neutrons is developed on a cylinder sample, and an empirical formula for scattered neutrons is obtained. According to the results given by Monte Carlo methods, the parameters in the empirical formula are obtained with curve fitting, which confirms the logicality of the empirical formula. The curve-fitted parameters of common materials such as 6 LiD are given. (authors)

  14. Inelastic scattering of 275 keV neutrons by silver

    International Nuclear Information System (INIS)

    Litvinsky, L.L.; Zhigalov, Ya.A.; Krivenko, V.G.; Purtov, O.A.; Sabbagh, S.

    1997-01-01

    Neutron total, elastic and inelastic scattering cross-scattering of Ag at the E n = 275 KeV neutron energy were measured by using the filtered neutron beam of the WWR-M reactor in Kiev. The d-neutron strength function S n2 of Ag was determined from the analysis of all available data in the E n ≤ keV energy region on neutron inelastic scattering cross-sections with excitation of the first isomeric levels I π m = 7/2 + , E m ∼ 90 keV of 107,109 Ag: S n2 = (1.03 ± 0.19) · 10 -4 . (author). 10 refs, 3 figs

  15. Some thoughts on the future of neutron scattering

    International Nuclear Information System (INIS)

    Egelstaff, P.A.

    1991-01-01

    Attendance of ICANS meetings believe that neutron scattering has a bright future, but critics of neutron scattering argue that its practitioners are an aging group, that they use a few, very expensive neutron sources and that the interesting science may be done by other techniques. The ICANS committee asked me to comment on the future of neutron scattering in the light of this contrast. Some comments will be made on the age distribution, on the proper distribution of sources, on the convenient availability of neutron instruments and methods, on the expansion into new areas of science, on applications to industry and on the probable impact of synchrotron sources. It is hoped that these comments will lead to an outward looking discussion on the future. (author)

  16. Set of thermal neutron-scattering experiments for the Weapons Neutron Research Facility

    International Nuclear Information System (INIS)

    Brugger, R.M.

    1975-12-01

    Six classes of experiments form the base of a program of thermal neutron scattering at the Weapons Neutron Research (WNR) Facility. Three classes are to determine the average microscopic positions of atoms in materials and three are to determine the microscopic vibrations of these atoms. The first three classes concern (a) powder sample neutron diffraction, (b) small angle scattering, and (c) single crystal Laue diffraction. The second three concern (d) small kappa inelastic scattering, (e) scattering surface phonon measurements, and (f) line widths. An instrument to couple with the WNR pulsed source is briefly outlined for each experiment

  17. The dynamics of physisorbed layers studied by neutron scattering

    International Nuclear Information System (INIS)

    Nielsen, M.; McTague, J.P.

    1978-01-01

    We discuss the neutron scattering technique applied to the study of adsorbed thin films. Despite the fact that neutrons are scattered very weakly by surfaces, recent studies have shown that both structural and dynamical information can be obtained even for submonolayer coverages. Results will be shown for films of Ar, D 2 , H 2 , and O 2 adsorbed on (001) surfaces of graphite and for H 2 molecules adsorbed on activated alumina. (orig.) [de

  18. Neutron scattering research at JAERI reactors - past, present and future -

    International Nuclear Information System (INIS)

    Funahashi, Satoru; Morii, Yukio; Minakawa, Nobuaki

    1992-01-01

    It was in 1961 that the first neutron scattering experiment was performed in Japan at JRR-2. The start of JRR-3 in 1964 accelerated the neutron scattering activities in Japan. The research in this field in Japan grew up by using these two research reactors. Among them JRR-2 has played an important role because its neutron flux was about seven times higher than that of the old JRR-3. The completion of the new JRR-3M in 1990 made an epoch to the neutron scattering activities in Japan. The long-waited JRR-3M came up to the expectations of the scientists of Japan. It is a realization of the ideal reactor with tangential beam holes, cold source and neutron guides in a large guide hall. The flux at the neutron scattering instruments is about five times higher than that of JRR-2. Utilization of JRR-3M has just started. Twelve neutron scattering machines are running there. The number will increase up to close twenty in a couple of years. (author)

  19. Small Angle Neutron Scattering instrument at Malaysian TRIGA reactor

    Energy Technology Data Exchange (ETDEWEB)

    Mohd, Shukri; Kassim, Razali; Mahmood, Zal Uyun [Malaysian Inst. for Nuclear Technology Research (MINT), Bangi, Kajang (Malaysia); Radiman, Shahidan

    1998-10-01

    The TRIGA MARK II Research reactor at the Malaysian Institute for Nuclear Research (MINT) was commissioned in July 1982. Since then various works have been performed to utilise the neutrons produced from this steady state reactor. One of the project involved the Small Angle Neutron Scattering (SANS). (author)

  20. A high pressure sample facility for neutron scattering

    International Nuclear Information System (INIS)

    Carlile, C.J.; Glossop, B.H.

    1981-06-01

    Commissioning tests involving deformation studies and tests to destruction as well as neutron diffraction measurements of a standard sample have been carried out on the SERC high pressure sample facility for neutron scattering studies. A detailed description of the pressurising equipment is given. (author)

  1. Spectrometer for neutron inelastic scattering investigations of microsamples

    International Nuclear Information System (INIS)

    Balagurov, A.M.; Kozlenko, D.P.; Platonov, S.L.; Savenko, B.N.; Glazkov, V.P.; Krasnikov, Yu.M.; Naumov, I.V.; Pukhov, A.V.; Somenkov, V.A.; Syrykh, G.F.

    1997-01-01

    A new neutron spectrometer for investigation of inelastic neutron scattering on polycrystal microsamples under high pressure in sapphire and diamond anvils cells is described. The spectrometer is operating at the IBR-2 pulsed reactor in JINR. Parameters and methodical peculiarities of the spectrometer and the examples of experimental studies are given. (author)

  2. Applications of neutron scattering to the study of magnetic materials

    International Nuclear Information System (INIS)

    Koehler, W.C.

    1976-01-01

    The types of interactions that neutrons undergo with condensed matter are reviewed and those properties of neutrons that make them an ideal probe for the study of magnetism on a microscopic scale are discussed. Following a very brief survey of experimental methods, a few illustrative examples of specific investigations are described in sufficient detail to illustrate the power of the techniques. Views as to the future directions that may be taken by neutron scattering are presented

  3. Neutron scattering: history, present state and perspectives

    International Nuclear Information System (INIS)

    Belushkin, A.V.

    1999-01-01

    The paper reminds some milestones in development of condensed matter research with neutrons. Present status of the investigations in this field is briefly outlined. An analysis is given on the situation and future prospects in different neutron sources development in Russia and in the world. The next generation neutron sources projects in Japan, USA and Europe are reviewed

  4. Collective Excitations in Liquid Hydrogen Observed by Coherent Neutron Scattering

    DEFF Research Database (Denmark)

    da Costa Carneiro, Kim; Nielsen, M.; McTague, J. P.

    1973-01-01

    Coherent scattering of neutrons by liquid parahydrogen shows the existence of well-defined collective excitations in this liquid. Qualitative similarity with the scattering from liquid helium is found. Furthermore, in the range of observed wave vectors, 0.7 Å-1 ≤κ≤3.1 Å-1, extending from the firs...

  5. Inelastic neutron scattering for materials science and engineering

    International Nuclear Information System (INIS)

    Shapiro, S.M.

    1995-01-01

    The neutron is the ideal probe for studying the positions and motions of atoms in condensed matter. The main advantage of the neutron in inelastic scattering results from its heavy mass when compared to other particles which are used to probe materials such as the photon (light, x-rays, or γ-rays) or the electron. The author discusses the application of neutron scattering to study a number of different materials related problems, including, hard magnets, shape memory effects, and hydrogen distribution in metals

  6. A combined neutron scattering and simulation study on bioprotectant systems

    Energy Technology Data Exchange (ETDEWEB)

    Affouard, F. [Laboratoire de Dynamique et Structure des Materiaux Moleculaires UMR 8024, Universite Lille I - 59655 Villeneuve d' Ascq cedex (France); Bordat, P. [Laboratoire de Dynamique et Structure des Materiaux Moleculaires UMR 8024, Universite Lille I - 59655 Villeneuve d' Ascq cedex (France); Descamps, M. [Laboratoire de Dynamique et Structure des Materiaux Moleculaires UMR 8024, Universite Lille I - 59655 Villeneuve d' Ascq cedex (France); Lerbret, A. [Laboratoire de Dynamique et Structure des Materiaux Moleculaires UMR 8024, Universite Lille I - 59655 Villeneuve d' Ascq cedex (France); Magazu, S. [Dipartimento di Fisica and INFM, Universita di Messina, P.O. Box 55, I-98166 Messina (Italy); Migliardo, F. [Laboratoire de Dynamique et Structure des Materiaux Moleculaires UMR 8024, Universite Lille I - 59655 Villeneuve d' Ascq cedex (France); Dipartimento di Fisica and INFM, Universita di Messina, P.O. Box 55, I-98166 Messina (Italy)], E-mail: fmigliardo@unime.it; Ramirez-Cuesta, A.J. [ISIS Facility, Rutherford Appleton Laboratory, Chilton, Didcot (United Kingdom); Telling, M.F.T. [ISIS Facility, Rutherford Appleton Laboratory, Chilton, Didcot (United Kingdom)

    2005-10-31

    The present work shows quasi elastic neutron scattering, neutron spin echo and inelastic neutron scattering results on a class of bioprotectant systems, such as homologous disaccharides (i.e., trehalose and sucrose)/water solutions, as a function of temperature. The whole set of findings indicates a noticeable 'kosmotrope' character of the disaccharides, and in particular of trehalose, which is able to strongly modify both the structural and dynamical properties of water. This superior capability of trehalose can be linked to its higher bioprotective effectiveness in respect with the other disaccharides.

  7. Superfluidity, Bose condensation and neutron scattering in liquid 4He

    International Nuclear Information System (INIS)

    Silver, R.N.

    1997-01-01

    The relation between superfluidity and Bose condensation in 4 He provides lessons that may be valuable in understanding the strongly correlated electron system of high T c superconductivity. Direct observation of a Bose condensate in the superfluid by deep inelastic neutron scattering measurements has been attempted over many years. But the impulse approximation, which relates momentum distributions to neutron scattering structure functions, is broadened by final state effects. Nevertheless, the excellent quantitative agreement between ab initio quantum many body theory and high precision neutron experiments provides confidence in the connection between superfluidity and Bose condensation

  8. Introduction of sample environment equipment for neutron scattering experiments

    International Nuclear Information System (INIS)

    Shimojo, Yutaka; Ihata, Yoshiaki; Kaneko, Koji; Takeda, Masayasu

    2013-02-01

    Neutron scattering experiments have been frequently performed under variety of sample conditions, such as various temperatures, pressures, magnetic fields and stresses, and those complex conditions to fully utilize superior properties of neutron. To this aim, a number of sample environment equipment, refrigerators, furnaces, pressure cells, superconducting magnets are equipped in JRR-3 to be used for experiments. In this document, all available sample environment equipment in both JRR-3 reactor and guide halls are summarized. We hope this document would help neutron scattering users to perform effective and excellent experiments. (author)

  9. The hydrogen anomaly problem in neutron Compton scattering

    Science.gov (United States)

    Karlsson, Erik B.

    2018-03-01

    Neutron Compton scattering (also called ‘deep inelastic scattering of neutrons’, DINS) is a method used to study momentum distributions of light atoms in solids and liquids. It has been employed extensively since the start-up of intense pulsed neutron sources about 25 years ago. The information lies primarily in the width and shape of the Compton profile and not in the absolute intensity of the Compton peaks. It was therefore not immediately recognized that the relative intensities of Compton peaks arising from scattering on different isotopes did not always agree with values expected from standard neutron cross-section tables. The discrepancies were particularly large for scattering on protons, a phenomenon that became known as ‘the hydrogen anomaly problem’. The present paper is a review of the discovery, experimental tests to prove or disprove the existence of the hydrogen anomaly and discussions concerning its origin. It covers a twenty-year-long history of experimentation, theoretical treatments and discussions. The problem is of fundamental interest, since it involves quantum phenomena on the subfemtosecond time scale, which are not visible in conventional thermal neutron scattering but are important in Compton scattering where neutrons have two orders of magnitude times higher energy. Different H-containing systems show different cross-section deficiencies and when the scattering processes are followed on the femtosecond time scale the cross-section losses disappear on different characteristic time scales for each H-environment. The last section of this review reproduces results from published papers based on quantum interference in scattering on identical particles (proton or deuteron pairs or clusters), which have given a quantitative theoretical explanation both regarding the H-cross-section reduction and its time dependence. Some new explanations are added and the concluding chapter summarizes the conditions for observing the specific quantum

  10. Fast Neutron Elastic and Inelastic Scattering of Vanadium

    Energy Technology Data Exchange (ETDEWEB)

    Holmqvist, B; Johansson, S G; Lodin, G; Wiedling, T

    1969-11-15

    Fast neutron scattering interactions with vanadium were studied using time-of-flight techniques at several energies in the interval 1.5 to 8.1 MeV. The experimental differential elastic scattering cross sections have been fitted to optical model calculations and the inelastic scattering cross sections have been compared with Hauser-Feshbach calculations, corrected for the fluctuation of compound-nuclear level widths.

  11. The world’s first pelletized cold neutron moderator at a neutron scattering facility

    Energy Technology Data Exchange (ETDEWEB)

    Ananiev, V.; Belyakov, A.; Bulavin, M.; Kulagin, E.; Kulikov, S.; Mukhin, K.; Petukhova, T.; Sirotin, A.; Shabalin, D.; Shabalin, E.; Shirokov, V.; Verhoglyadov, A., E-mail: verhoglyadov_al@mail.ru

    2014-02-01

    In July 10, 2012 cold neutrons were generated for the first time with the unique pelletized cold neutron moderator CM-202 at the IBR-2M reactor. This new moderator system uses small spherical beads of a solid mixture of aromatic hydrocarbons (benzene derivatives) as the moderating material. Aromatic hydrocarbons are known as the most radiation-resistant hydrogenous substances and have properties to moderate slow neutrons effectively. Since the new moderator was put into routine operation in September 2013, the IBR-2 research reactor of the Frank Laboratory of Neutron Physics has consolidated its position among the world’s leading pulsed neutron sources for investigation of matter with neutron scattering methods.

  12. Small Angle Neutron Scattering From Iron. Vol. 2

    Energy Technology Data Exchange (ETDEWEB)

    Adib, M; Abdel-Kawy, A; Naguib, K; Habib, N; Kilany, M [Reactor and Neutron Physics Dept., Nuclear Research Centre, AEA, Cairo, (Egypt); Wahba, M [Faculty of Engineering, ain Shams University, Cairo, (Egypt); Ashry, A [Faculty of Education, Ain Shams University, Cairo, (Egypt)

    1996-03-01

    The total neutron cross-section measurements have been carried out for iron in both metallic and powder forms in the wavelengths band 0.35 nm to 0.52 nm. The measurements were performed using the TOF spectrometer installed in front of one of the horizontal channels of the ET-RR-1 reactor. The observed behavior for the small-angle neutron scattering cross-section of iron powder was analyzed in terms of its particle diameter, incident neutron wavelength and beam divergence. It was found that for iron particles of diameter 25 {mu}m the small-angle neutron scattering is only due to refraction of neutron wave traversing the particles. A method was established to determine the particle size of iron powders within an accuracy of 8% which is higher than that obtained by mesh analysis. 4 figs., 1 tab.

  13. Methyl group rotation and segmental motion in atactic polypropylene. An incoherent quasi elastic neutron scattering investigation

    International Nuclear Information System (INIS)

    Arrighi, V.; Triolo, A.

    1999-01-01

    Complete text of publication follows. Results from the analysis of recent quasielastic neutron scattering (QENS) experiments on atactic polypropylene (aPP), are presented both in the sub-T g and above T g regimes. Experiments were carried out on the IRIS (ISIS, Rutherford Appleton Laboratory, UK) and IN10 (ILL FR) spectrometers in the temperature range from 140 to 400 K. Different instrumental resolutions were used in order to cover a wide energy window. The high resolution data collected on IN10 using the fixed energy scan technique, give clear evidence of two separate dynamic processes that we attribute to methyl group rotational hopping (below T g ) and to segmental motion (above T g ), respectively. Data were fitted using a model involving a distribution of relaxation rates. The IN10 results are used in interpreting and analyzing the QENS data from the IRIS spectrometer. In order to exploit the different energy resolutions of IRIS, Fourier inversion of the experimental data was carried out. This approach to data analysis allows us to widen the energy range available for data analysis. Due to the high activation energy of the methyl group hopping in aPP, this motion overlaps with the segmental relaxation, thus making analysis of high temperature data quite complex. The IN10 results are employed in order to perform data analysis in terms of two distinct processes. (author)

  14. New era of neutron scattering research on advanced materials

    International Nuclear Information System (INIS)

    Ikeda, Susumu

    2001-01-01

    The projects of the next generation of pulsed spallation neutron source are planed in USA, Europe and Japan. They are one order of magnitude more powerful than the most powerful existing neutron source, ISIS in UK. They offer the exciting prospects for the future, and will open the new era of neutron scattering research on advanced materials. The Japanese project is named as the 'Joint project' between JAERI and KEK on high-intensity proton accelerators. The details of the neutron science facility in the 'Joint project' and the sciences to be developed are summarized. (author)

  15. Neutron polarization in polarized 3He targets

    International Nuclear Information System (INIS)

    Friar, J.L.; Gibson, B.F.; Payne, G.L.; Bernstein, A.M.; Chupp, T.E.

    1990-01-01

    Simple formulas for the neutron and proton polarizations in polarized 3 He targets are derived assuming (1) quasielastic final states; (2) no final-state interactions; (3) no meson-exchange currents; (4) large momentum transfers; (5) factorizability of 3 He SU(4) response-function components. Numerical results from a wide variety of bound-state solutions of the Faddeev equations are presented. It is found that this simple model predicts the polarization of neutrons in a fully polarized 3 He target to be 87%, while protons should have a slight residual polarization of -2.7%. Numerical studies show that this model works very well for quasielastic electron scattering

  16. 2010 American Conference on Neutron Scattering (ACNS 2010)

    Energy Technology Data Exchange (ETDEWEB)

    Billinge, Simon

    2011-06-17

    The ACNS provides a focal point for the national neutron user community to strengthen ties within this diverse group, while at the same time promoting neutron research among colleagues in related disciplines identified as “would-be” neutron users. The American Conference on Neutron Scattering thus serves a dual role as a national user meeting and a scientific meeting. As a venue for scientific exchange, the ACNS showcases recent results and provides forums for scientific discussion of neutron research in diverse fields such as hard and soft condensed matter, liquids, biology, magnetism, engineering materials, chemical spectroscopy, crystal structure, and elementary excitations, fundamental physics and development of neutron instrumentation through a combination of invited talks, contributed talks and poster sessions. As a “super-user” meeting, the ACNS fulfills the main objectives of users' meetings previously held periodically at individual national neutron facilities, with the advantage of a larger and more diverse audience. To this end, each of the major national neutron facilities (NIST, LANSCE, HFIR and SNS) have an opportunity to exchange information and update users, and potential users, of their facility. This is also an appropriate forum for users to raise issues that relate to the facilities. For many of the national facilities, this super-user meeting should obviate the need for separate user meetings that tax the time, energy and budgets of facility staff and the users alike, at least in years when the ACNS is held. We rely upon strong participation from the national facilities. The NSSA intends that the American Conference on Neutron Scattering (ACNS) will occur approximately every two years, but not in years that coincide with the International or European Conferences on Neutron Scattering. The ACNS is to be held in association with one of the national neutron centers in a rotating sequence, with the host facility providing local

  17. Data acquisition system for the neutron scattering instruments at the intense pulsed neutron source

    International Nuclear Information System (INIS)

    Crawford, R.K.; Daly, R.T.; Haumann, J.R.; Hitterman, R.L.; Morgan, C.B.; Ostrowski, G.E.; Worlton, T.G.

    1981-01-01

    The Intense Pulsed Neutron Source (IPNS) at Argonne National Laboratory is a major new user-oriented facility which is now coming on line for basic research in neutron scattering and neutron radiation damage. This paper describes the data-acquisition system which will handle data acquisition and instrument control for the time-of-flight neutron-scattering instruments at IPNS. This discussion covers the scientific and operational requirements for this system, and the system architecture that was chosen to satisfy these requirements. It also provides an overview of the current system implementation including brief descriptions of the hardware and software which have been developed

  18. Experimental studies of the critical scattering of neutrons for large scattering vectors

    International Nuclear Information System (INIS)

    Ciszewski, R.

    1972-01-01

    The most recent results concerned with the critical scattering of neutrons are reviewed. The emphasis is on the so-called thermal shift, that is the shift of the main maximum in the intensity of critically scattered neutrons with temperature changes. Four theories of this phenomenon are described and their shortcomings are shown. It has been concluded that the situation is involved at present and needs further theoretical and experimental study. (S.B.)

  19. Earth formation pulsed neutron porosity logging system utilizing epithermal neutron and inelastic scattering gamma ray detectors

    International Nuclear Information System (INIS)

    Smith, H.D. Jr.; Smith, M.P.; Schultz, W.E.

    1978-01-01

    An improved pulsed neutron porosity logging system is provided in the present invention. A logging tool provided with a 14 MeV pulsed neutron source, an epithermal neutron detector and an inelastic scattering gamma ray detector is moved through a borehole. The detection of inelastic gamma rays provides a measure of the fast neutron population in the vicinity of the detector. repetitive bursts of neutrons irradiate the earth formation and, during the busts, inelastic gamma rays representative of the fast neutron population is sampled. During the interval between bursts the epithermal neutron population is sampled along with background gamma radiation due to lingering thermal neutrons. the fast and epithermal neutron population measurements are combined to provide a measurement of formation porosity

  20. Toward a new polyethylene scattering law determined using inelastic neutron scattering

    International Nuclear Information System (INIS)

    Lavelle, C.M.; Liu, C.-Y.; Stone, M.B.

    2013-01-01

    Monte Carlo neutron transport codes such as MCNP rely on accurate data for nuclear physics cross-sections to produce accurate results. At low energy, this takes the form of scattering laws based on the dynamic structure factor, S(Q,E). High density polyethylene (HDPE) is frequently employed as a neutron moderator at both high and low temperatures, however the only cross-sections available are for ambient temperatures (∼300K), and the evaluation has not been updated in quite some time. In this paper we describe inelastic neutron scattering measurements on HDPE at 5 and 294 K which are used to improve the scattering law for HDPE. We review some of the past HDPE scattering laws, describe the experimental methods, and compare computations using these models to the measured S(Q,E). The total cross-section is compared to available data, and the treatment of the carbon secondary scatterer as a free gas is assessed. We also discuss the use of the measurement itself as a scattering law via the one phonon approximation. We show that a scattering law computed using a more detailed model for the Generalized Density of States (GDOS) compares more favorably to this experiment, suggesting that inelastic neutron scattering can play an important role in both the development and validation of new scattering laws for Monte Carlo work. -- Highlights: ► Polyethylene at 5 K and 300 K is measured using inelastic neutron scattering (INS). ► Measurements conducted at the Wide Angular-Range Chopper Spectrometer at SNS. ► Several models for Polyethylene are compared to measurements. ► Improvements to existing models for the polyethylene scattering law are suggested. ► INS is shown to be highly valuable tool for scattering law development

  1. Status of thermal neutron scattering data for graphite

    International Nuclear Information System (INIS)

    Mattes, M.; Keinert, J.

    2005-07-01

    At thermal neutron energies, the binding of the scattering nucleus in a solid, liquid, or gas affects the cross sections and the angular and energy distributions of the scattered neutrons. These effects are described in the thermal sub-library of evaluated files in File 7 of the ENDF-6 format. A re-evaluation of thermal neutron scattering data for carbon bound in graphite has been performed to investigate the impact of models (e.g., generalised frequency distributions) based on different experimental and theoretical data for the generation of scattering law data files S(α,β,T) and coherent elastic scattering data. Two phonon frequency distributions of graphite published in 2002 and 2004 were considered and the results compared with those based on the phonon spectra from Koppel et al. (published in 1968), on which the evaluations of ENDF/B-VI and JEFF-3.1 are based. The new frequency distributions were partly derived from ab initio simulations. Detailed comparisons with measurements of differential and integral neutron cross sections and other relevant data are reported. In addition, thermal MCNP data sets for use in the continuous Monte Carlo codes MCNP and MCNPX were generated from these evaluations for different temperatures. Calculated neutron spectra were found to be in good agreement with the measurements. (author)

  2. Neutron scattering at the high-flux isotope reactor

    International Nuclear Information System (INIS)

    Cable, J.W. Chakoumakos, B.C.; Dai, P.

    1995-01-01

    The title facilities offer the brightest source of neutrons in the national user program. Neutron scattering experiments probe the structure and dynamics of materials in unique and complementary ways as compared to x-ray scattering methods and provide fundamental data on materials of interest to solid state physicists, chemists, biologists, polymer scientists, colloid scientists, mineralogists, and metallurgists. Instrumentation at the High- Flux Isotope Reactor includes triple-axis spectrometers for inelastic scattering experiments, a single-crystal four diffractometer for crystal structural studies, a high-resolution powder diffractometer for nuclear and magnetic structure studies, a wide-angle diffractometer for dynamic powder studies and measurements of diffuse scattering in crystals, a small-angle neutron scattering (SANS) instrument used primarily to study structure-function relationships in polymers and biological macromolecules, a neutron reflectometer for studies of surface and thin-film structures, and residual stress instrumentation for determining macro- and micro-stresses in structural metals and ceramics. Research highlights of these areas will illustrate the current state of neutron science to study the physical properties of materials

  3. Critical magnetic scattering of polarized neutrons on iron

    International Nuclear Information System (INIS)

    Hetzelt, M.

    1975-01-01

    A new spectrometer has been built and tested. The instrument was designed particularly for small angle scattering of polarized neutrons whereby the degree of polarisation of the scattered neutrons can be measured. The use of polarizing neutron pipes as polarizer and analyser allows the performence with a very broad wavelength spectrum (2 A 7 n/cm 2 sec) with good collimation (Δ theta approximately 0.2 0 ). The instrument is applied for the measurement of the critical magnetic scattering of polarized neutrons on an iron single crystal. For this purpose a special oven with an appropriate magnetic field configuration and a high precision in temperature has been constructed. The measured intensity distributions are in good agreement with other experiments. The critical exponent of the correlation range xi results in 0.65 +- 0.06. Angle and temperature dependence of the scattered neutron polarisation could be determined with good precision. The measurements are partly in extreme contradiction to the only hitherto existing experiment of this kind of Drabkin et al, and to assumptions in the theoretical evaluation. This contradiction is shown to be caused by the influence of multiple scattering. (orig./HPOE) [de

  4. Development of High Spectral Resolution Technique for Registration Quasielastic Light Scattering Spectra Including Rayleigh and Brillouin Scattering as a Diagnostic Tool in Materials Characterization

    National Research Council Canada - National Science Library

    Bairamov, Bakhysh

    2004-01-01

    ...: As detailed in an on-line proposal the contractor will: 1) develop and build an optical device, fitted to a Fabry-Perot interferometer, to perform high-resolution quasieleastic light scattering spectroscopy; 2...

  5. Development of new methods for studying nanostructures using neutron scattering

    International Nuclear Information System (INIS)

    Pynn, Roger

    2016-01-01

    The goal of this project was to develop improved instrumentation for studying the microscopic structures of materials using neutron scattering. Neutron scattering has a number of advantages for studying material structure but suffers from the well-known disadvantage that neutrons' ability to resolve structural details is usually limited by the strength of available neutron sources. We aimed to overcome this disadvantage using a new experimental technique, called Spin Echo Scattering Angle Encoding (SESAME) that makes use of the neutron's magnetism. Our goal was to show that this innovation will allow the country to make better use of the significant investment it has recently made in a new neutron source at Oak Ridge National Laboratory (ORNL) and will lead to increases in scientific knowledge that contribute to the Nation's technological infrastructure and ability to develop advanced materials and technologies. We were successful in demonstrating the technical effectiveness of the new method and established a baseline of knowledge that has allowed ORNL to start a project to implement the method on one of its neutron beam lines.

  6. Background determination for the neutron-neutron scattering experiment at the reactor YAGUAR

    Energy Technology Data Exchange (ETDEWEB)

    Muzichka, A.Yu. [Joint Institute for Nuclear Research, 141980 Dubna (Russian Federation); Furman, W.I. [Joint Institute for Nuclear Research, 141980 Dubna (Russian Federation); Lychagin, E.V. [Joint Institute for Nuclear Research, 141980 Dubna (Russian Federation); Krylov, A.R. [Joint Institute for Nuclear Research, 141980 Dubna (Russian Federation); Nekhaev, G.V. [Joint Institute for Nuclear Research, 141980 Dubna (Russian Federation); Sharapov, E.I. [Joint Institute for Nuclear Research, 141980 Dubna (Russian Federation); Shvetsov, V.N. [Joint Institute for Nuclear Research, 141980 Dubna (Russian Federation); Strelkov, A.V. [Joint Institute for Nuclear Research, 141980 Dubna (Russian Federation); Levakov, B.G. [Russian Federal Nuclear Center-All-Russian Research Institute of Technical Physics, PO Box 245, 456770 Snezhinsk (Russian Federation); Lyzhin, A.E. [Russian Federal Nuclear Center-All-Russian Research Institute of Technical Physics, PO Box 245, 456770 Snezhinsk (Russian Federation); Chernukhin, Yu.I. [Russian Federal Nuclear Center-All-Russian Research Institute of Technical Physics, PO Box 245, 456770 Snezhinsk (Russian Federation); Kandiev, Ya.Z. [Russian Federal Nuclear Center-All-Russian Research Institute of Technical Physics, PO Box 245, 456770 Snezhinsk (Russian Federation); Howell, C.R. [Duke University and Triangle Universities Nuclear Laboratory, Durham, NC 27708-0308 (United States); Mitchell, G.E. [North Carolina State University, Raleigh, NC 27695-8202 (United States); Triangle Universities Nuclear Laboratory, Durham, NC 27708-0308 (United States); Crawford, B.E. [Gettysburg College, Box 405, Gettysburg, PA 17325 (United States); Stephenson, S.L. [Gettysburg College, Box 405, Gettysburg, PA 17325 (United States)]. E-mail: sstephen@gettysburg.edu; Tornow, W. [Duke University and Triangle Universities Nuclear Laboratory, Durham, NC 27708-0308 (United States)

    2007-06-01

    The motivation and design is outlined for the experiment to measure the neutron-neutron singlet scattering length directly with thermal neutrons at the pulsed reactor YAGUAR. A statistical accuracy of 3% can be reached, though achieving the goal of an overall accuracy of 3-5% for the nn-scattering length depends on the background level. Possible sources of background are discussed in depth and the results of extensive modeling of the background are presented. Measurements performed at YAGUAR to test these background calculations are described. The experimental results indicate an anticipated background level up to 30% relative to the expected nn effect at the maximal energy burst of the reactor. The conclusion is made that the nn experiment at YAGUAR is feasible to produce the first directly measured value for the neutron-neutron scattering length.

  7. Small angle neutron scattering and small angle X-ray scattering ...

    Indian Academy of Sciences (India)

    Abstract. The morphology of carbon nanofoam samples comprising platinum nanopar- ticles dispersed in the matrix was characterized by small angle neutron scattering (SANS) and small angle X-ray scattering (SAXS) techniques. Results show that the structure of pores of carbon matrix exhibits a mass (pore) fractal nature ...

  8. Investigation of collective excitations in fluid neon by coherent neutron scattering at small scattering vectors

    International Nuclear Information System (INIS)

    Bell, H.G.

    1976-07-01

    The energy spectra of Ne studied under different temperatures and pressures with the aid of inelastic, coherent neutron scattering can be described by a scattering law derived from the basic hydrodynamic equations. The Brillouin lines found with very small momentum transfer 0.06 A -1 -1 are interpreted as collective, adiabatic pressure fluctuations. (orig./WL) [de

  9. Monte Carlo simulation of fast neutron scattering experiments including DD-breakup neutrons

    Energy Technology Data Exchange (ETDEWEB)

    Schmidt, D.; Siebert, B.R.L.

    1993-06-01

    The computational simulation of the deuteron breakup in a scattering experiment has been investigated. Experimental breakup spectra measured at 16 deuteron energies and at 7 angles for each energy served as the data base. Analysis of these input data and of the conditions of the scattering experiment made it possible to reduce the input data. The use of one weighted breakup spectrum is sufficient to simulate the scattering spectra at one incident neutron energy. A number of tests were carried out to prove the validity of this result. The simulation of neutron scattering on carbon, including the breakup, was compared with measured spectra. Differences between calculated and measured spectra were for the most part within the experimental uncertainties. Certain significant deviations can be attributed to erroneous scattering cross sections taken from an evaluation and used in the simulation. Scattering on higher-lying states in [sup 12]C can be analyzed by subtracting the simulated breakup-scattering from the experimental spectra. (orig.)

  10. Monte Carlo simulation of fast neutron scattering experiments including DD-breakup neutrons

    International Nuclear Information System (INIS)

    Schmidt, D.; Siebert, B.R.L.

    1993-06-01

    The computational simulation of the deuteron breakup in a scattering experiment has been investigated. Experimental breakup spectra measured at 16 deuteron energies and at 7 angles for each energy served as the data base. Analysis of these input data and of the conditions of the scattering experiment made it possible to reduce the input data. The use of one weighted breakup spectrum is sufficient to simulate the scattering spectra at one incident neutron energy. A number of tests were carried out to prove the validity of this result. The simulation of neutron scattering on carbon, including the breakup, was compared with measured spectra. Differences between calculated and measured spectra were for the most part within the experimental uncertainties. Certain significant deviations can be attributed to erroneous scattering cross sections taken from an evaluation and used in the simulation. Scattering on higher-lying states in 12 C can be analyzed by subtracting the simulated breakup-scattering from the experimental spectra. (orig.)

  11. Study on lattice relaxation type transformation of (CuNi)sub(3-x) Alsub(1+x) alloy by inelastic neutron scattering

    International Nuclear Information System (INIS)

    Kajitani, Tsuyoshi; Hirano, Ken-ichi

    1975-01-01

    Inelastic scattering experiment was carried out on (Cu Ni)sub(3-x)Alsub(1+x) alloy at room temperature. The sample was annealed in vacuum for two hours at 950 0 C, quenched in water at 0 0 C, and aged for about one year. The energy spectrum of scattered neutrons was measured by T-O-F method. The measurement was performed for phonons at reciprocal lattice point (2/3--3/4, 2/3--3/4, 0) corresponding to the period of static shearing deformation. The up-scattering peak (Pq 1) observed at 2 theta = 38 0 in case of -14.5 0 of incident beam direction has width of 14.8 MeV, and is not considered to be a coherent inelastic scattering peak. The up-scattering peak (Pq 2) of 9 0 of incident beam direction has width of 17.3 MeV. The peak Pq 1 is considered as quasi-elastic scattering. The reflection point in the reciprocal lattice space of elastic scattering waves at 2 theta = 38 0 in case of -14.5 0 incident angle is near the [1 1 1] reciprocal lattice point of DO 3 structure. In case of 9 0 incident angle, it is near the [1 0 0] point. As conclusions, (1) it is not said that only the shear waves on the axis are freezed in the martensite transformation of (CuNi)sub(3-x)Alsub(1+x) alloy, (2) an L mode quasi-elastic peak is seen near the [1 1 1] reciprocal lattice point, (3) a T mode phonon peak is observed near the [1 1 0] reciprocal lattice point, and (4) T mode phonons are seen near [1/2, 1/2, 1/2]. (Kato, T.)

  12. Fragility of complexity biophysical systems by neutron scattering

    Energy Technology Data Exchange (ETDEWEB)

    Magazu, Salvatore [Dipartimento di Fisica, Universita di Messina, P.O. Box 55, I-98166 Messina (Italy)]. E-mail: smagazu@unime.it; Migliardo, Federica [Dipartimento di Fisica, Universita di Messina, P.O. Box 55, I-98166 Messina (Italy); Bellocco, Ersilia [Dipartimento di Chimica Organica e Biologica, Universita di Messina, I-98166 Messina (Italy); Lagana, Giuseppina [Dipartimento di Chimica Organica e Biologica, Universita di Messina, I-98166 Messina (Italy); Mondelli, Claudia [CNR-INFM OGG and CRS-SOFT, c/o ILL, 6 Jules Horowitz, BP 156, 38042 Grenoble Cedex 9 (France)

    2006-11-15

    Neutron scattering is an exceptional tool to investigate structural and dynamical properties of systems of biophysical interest, such as proteins, enzymes, lipids and sugars. Moreover, elastic neutron scattering enhances the investigation of atomic motions in hydrated proteins in a wide temperature range and on the picosecond timescale. Homologous disaccharides, such as trehalose, maltose and sucrose, are cryptobiotic substances, since they allow to many organisms to undergo in a 'suspended life' state, known as cryptobiosis in extreme environmental conditions. The present paper is aimed to discuss the fragility degree of disaccharides, as evaluated of the temperature dependence of the mean square displacement by elastic neutron scattering, in order to link this feature with their bioprotective functions.

  13. Software for simulation and design of neutron scattering instrumentation

    DEFF Research Database (Denmark)

    Bertelsen, Mads

    designed using the software. The Union components uses a new approach to simulation of samples in McStas. The properties of a sample are split into geometrical and material, simplifying user input, and allowing the construction of complicated geometries such as sample environments. Multiple scattering...... from conventional choices. Simulation of neutron scattering instrumentation is used when designing instrumentation, but also to understand instrumental effects on the measured scattering data. The Monte Carlo ray-tracing package McStas is among the most popular, capable of simulating the path of each...... neutron through the instrument using an easy to learn language. The subject of the defended thesis is contributions to the McStas language in the form of the software package guide_bot and the Union components.The guide_bot package simplifies the process of optimizing neutron guides by writing the Mc...

  14. Neutron scattering in soft matter physics and chemistry

    International Nuclear Information System (INIS)

    White, J.W.

    1999-01-01

    Recent experiments area of soft matter science show that self assembly on the micron scale as well as the nanometer scale can be directed chemically. This lecture illustrates how such processes can be studied using the contrast variation available in neutron scattering through isotopic replacement and the techniques of neutron small angle scattering and neutron reflectivity. Related dynamical information at nanometer resolution and on time scales between a nanosecond and a few tenths of a picosecond will become accessible with brighter neutron sources. The examples presented concern the template induced crystallisation of zeolites, the liquid crystal template induced synthesis of mesoporous materials and the structure of thin films at the air water interface. (J.P.N.)

  15. Spin dynamics above the Curie temperature studied by neutron scattering

    International Nuclear Information System (INIS)

    Steinsvoll, O.; Riste, T.

    1986-01-01

    Neutron scattering can in principle give information about magnetic fluctuations over the entire atomic space and time domain. The weakness of the neutron-matter interaction renders this information undistorted by the neutron probe, but at the same time puts intensity limitations on the method. A considerable number of studies on the magnetism of 3d metals have been performed at some of the larger reactor laboratories. In the regions of overlap the experimental results from the different laboratories are consistent, but the interpretations are along different lines. Among the controversial issues are itinerancy versus localization, the degree of order above T C . In our talk we shall give an introduction to the neutron scattering method, including some of the sophisticated polarized beam methods. In the rest of the talk we shall review recent experimental results and some of the theoretical models used in their interpretation. (orig.)

  16. Fluence-compensated down-scattered neutron imaging using the neutron imaging system at the National Ignition Facility

    Energy Technology Data Exchange (ETDEWEB)

    Casey, D. T., E-mail: casey21@llnl.gov; Munro, D. H.; Grim, G. P.; Landen, O. L.; Spears, B. K.; Fittinghoff, D. N.; Field, J. E.; Smalyuk, V. A. [Lawrence Livermore National Laboratory, Livermore, California 94550 (United States); Volegov, P. L.; Merrill, F. E. [Los Alamos National Laboratory, Los Alamos, New Mexico 87545 (United States)

    2016-11-15

    The Neutron Imaging System at the National Ignition Facility is used to observe the primary ∼14 MeV neutrons from the hotspot and down-scattered neutrons (6-12 MeV) from the assembled shell. Due to the strong spatial dependence of the primary neutron fluence through the dense shell, the down-scattered image is convolved with the primary-neutron fluence much like a backlighter profile. Using a characteristic scattering angle assumption, we estimate the primary neutron fluence and compensate the down-scattered image, which reveals information about asymmetry that is otherwise difficult to extract without invoking complicated models.

  17. Some Notes on Neutron Up-Scattering and the Doppler-Broadening of High-Z Scattering Resonances

    Energy Technology Data Exchange (ETDEWEB)

    Parsons, Donald Kent [Los Alamos National Lab. (LANL), Los Alamos, NM (United States)

    2017-09-28

    When neutrons are scattered by target nuclei at elevated temperatures, it is entirely possible that the neutron will actually gain energy (i.e., up-scatter) from the interaction. This phenomenon is in addition to the more usual case of the neutron losing energy (i.e., down-scatter). Furthermore, the motion of the target nuclei can also cause extended neutron down-scattering, i.e., the neutrons can and do scatter to energies lower than predicted by the simple asymptotic models. In recent years, more attention has been given to temperature-dependent scattering cross sections for materials in neutron multiplying systems. This has led to the inclusion of neutron up-scatter in deterministic codes like Partisn and to free gas scattering models for material temperature effects in Monte Carlo codes like MCNP and cross section processing codes like NJOY. The free gas scattering models have the effect of Doppler Broadening the scattering cross section output spectra in energy and angle. The current state of Doppler-Broadening numerical techniques used at Los Alamos for scattering resonances will be reviewed, and suggestions will be made for further developments. The focus will be on the free gas scattering models currently in use and the development of new models to include high-Z resonance scattering effects. These models change the neutron up-scattering behavior.

  18. High energy neutron recoil scattering from liquid 4He

    International Nuclear Information System (INIS)

    Holt, R.S.; Needham, L.M.; Paoli, M.P.

    1987-10-01

    The neutron recoil scattering from liquid 4 He at 4.2 K and 1.6 K has been observed for a momentum transfer of 150 A -1 using the Electron Volt Spectrometer on the pulsed neutron source, ISIS. The experiment yielded mean atomic kinetic energy values = 14.8 +- 3 K at 4.2 K and = 14.6 +- 3.2 K at 1.6 K in good agreement with values obtained at lower momentum transfers. (author)

  19. Inelastic scattering of neutrons by spin waves in terbium

    DEFF Research Database (Denmark)

    Bjerrum Møller, Hans; Houmann, Jens Christian Gylden

    1966-01-01

    Measurements of spin-wave dispersion relations for magnons propagating in symmetry directions in ferromagnetic Tb; it is first experiment to give detailed information on magnetic excitations in heavy rare earths; Tb was chosen for these measurements because it is one of few rare-earth metals which...... does not have very high thermal-neutron capture cross section, so that inelastic neutron scattering experiments can give satisfactory information on magnon dispersion relations....

  20. Thermal neutron scattering studies of condensed matter under high pressures

    International Nuclear Information System (INIS)

    Carlile, C.J.; Salter, D.C.

    1978-01-01

    Although temperature has been used as a thermodynamic variable for samples in thermal neutron scattering experiments since the inception of the neutron technique, it is only in the last decade that high pressures have been utilised for this purpose. In the paper the problems particular to this field of work are outlined and a review is made of the types of high-pressure cells used and the scientific results obtained from the experiments. 103 references. (author)