DEFF Research Database (Denmark)
Kawasaki, Yu; Gavilano, Jorge L.; Keller, Lukas
2011-01-01
,0,1), independent of external magnetic fields for fields below a critical value H-c(T). The ordered moments of 2.18 mu(B) per Co ion are aligned along the crystallographic c axis. Within the screw chains, along the c axis, the moments are arranged antiferromagnetically. In the basal planes the spins are arranged......We report a neutron diffraction and muon spin relaxation mu SR study of static and dynamical magnetic properties of BaCo2V2O8, a quasi-one-dimensional spin-chain system. A proposed model for the antiferromagnetic structure includes: a propagation vector (k) over right arrow (AF) = (0...
Inami, T; Tanaka, H
1997-01-01
The spin dynamics of the hexagonal ABX sub 3 -type quasi-one-dimensional antiferromagnet CsVCl sub 3 is investigated by means of an inelastic neutron scattering technique. In good qualitative agreement with a recent spin-wave calculation including higher-order terms, a large scattering cross-section arising from two-magnon excitations is observed at the one-dimensional antiferromagnetic zone centre. In addition, we measured spin-wave excitations between the chains precisely and revealed that the spin-wave dispersion curves are modified in energy and in intensity on account of the anticrossing between the one-magnon branches and two-magnon continuum. These results demonstrate that anharmonic terms are important in the spin dynamics of CsVCl sub 3 even at low temperatures. We also measured the temperature dependence of the magnetic excitations and found that far above the Neel temperature the two-magnon process gives a considerable contribution to the inelastic spectrum. (author)
NMR relaxation rate in quasi one-dimensional antiferromagnets
Capponi, Sylvain; Dupont, Maxime; Laflorencie, Nicolas; Sengupta, Pinaki; Shao, Hui; Sandvik, Anders W.
We compare results of different numerical approaches to compute the NMR relaxation rate 1 /T1 in quasi one-dimensional (1d) antiferromagnets. In the purely 1d regime, recent numerical simulations using DMRG have provided the full crossover behavior from classical regime at high temperature to universal Tomonaga-Luttinger liquid at low-energy (in the gapless case) or activated behavior (in the gapped case). For quasi 1d models, we can use mean-field approaches to reduce the problem to a 1d one that can be studied using DMRG. But in some cases, we can also simulate the full microscopic model using quantum Monte-Carlo techniques. This allows to compute dynamical correlations in imaginary time and we will discuss recent advances to perform stochastic analytic continuation to get real frequency spectra. Finally, we connect our results to experiments on various quasi 1d materials.
A mean field study of the quasi-one-dimensional antiferromagnetic anisotropic Heisenberg model
International Nuclear Information System (INIS)
Benyoussef, A.
1996-10-01
The effect of the chain and the dimer anisotropies on the ground state energy and the energy gap of the spin-1/2 quasi-one-dimensional antiferromagnetic Heisenberg model is investigated using a mean field theory. The dependence of the magnetization and the effective hopping parameters on the anisotropy α xy (=J xy perpendicular /J xy parallel ) are presented for several values of the chain anisotropy. However, such a system exhibits a transition from antiferromagnetic ordered to disordered phases for arbitrary chain anisotropy and dimer anisotropy. (author). 22 refs, 11 figs
International Nuclear Information System (INIS)
Liu Juan-Juan; Wang Jin-Chen; Luo Wei; Sheng Jie-Ming; Bao Wei; He Zhang-Zhen; Danilkin, S. A.
2016-01-01
The magnetic structure of the spin-chain antiferromagnet SrCo_2V2O_8 is determined by single-crystal neutron diffraction experiment. The system undergoes a long-range magnetic order below the critical temperature T_N = 4.96 K. The moment of 2.16μ_B per Co at 1.6 K in the screw chain running along the c axis alternates in the c axis. The moments of neighboring screw chains are arranged antiferromagnetically along one in-plane axis and ferromagnetically along the other in-plane axis. This magnetic configuration breaks the four-fold symmetry of the tetragonal crystal structure and leads to two equally populated magnetic twins with the antiferromagnetic vector in the a or b axis. The very similar magnetic state to the isostructural BaCo_2V_2O_8 warrants SrCo_2V_2O_8 as another interesting half-integer spin-chain antiferromagnet for investigation on quantum antiferromagnetism. (paper)
Spinon confinement in a quasi-one-dimensional XXZ Heisenberg antiferromagnet
Lake, Bella; Bera, Anup K.; Essler, Fabian H. L.; Vanderstraeten, Laurens; Hubig, Claudius; Schollwock, Ulrich; Islam, A. T. M. Nazmul; Schneidewind, Astrid; Quintero-Castro, Diana L.
Half-integer spin Heisenberg chains constitute a key paradigm for quantum number fractionalization: flipping a spin creates a minimum of two elementary spinon excitations. These have been observed in numerous experiments. We report on inelastic neutron scattering experiments on the quasi-one-dimensional anisotropic spin-1/2 Heisenberg antiferromagnet SrCo2V2O8. These reveal a mechanism for temperature-induced spinon confinement, manifesting itself in the formation of sequences of spinon bound states. A theoretical description of this effect is achieved by a combination of analytical and numerical methods.
International Nuclear Information System (INIS)
Belik, A.A.; Azuma, M.; Takano, M.
2004-01-01
Properties of Sr 2 Cu(PO 4 ) 2 and Ba 2 Cu(PO 4 ) 2 having [Cu(PO 4 ) 2 ] ∞ linear chains in their structures with Cu-O-P-O-Cu linkages were studied by magnetic susceptibility (T=2-400 K, H=100 Oe) and specific heat measurements (T=0.45-21 K). Magnetic susceptibility versus temperature curves, χ(T), showed broad maxima at T M =92 K for Sr 2 Cu(PO 4 ) 2 and T M =82 K for Ba 2 Cu(PO 4 ) 2 characteristic of quasi-one-dimensional systems. The χ(T) data were excellently fitted by the spin susceptibility curve for the uniform S=1/2 chain (plus temperature-independent and Curie-Weiss terms) with g=2.153(4) and J/k B =143.6(2) K for Sr 2 Cu(PO 4 ) 2 and g=2.073(4) and J/k B =132.16(9) K for Ba 2 Cu(PO 4 ) 2 (Hamiltonian H=JΣS i S i+1 ). The similar J/k B values were obtained from the specific heat data. No anomaly was observed on the specific heat from 0.45 to 21 K for both compounds indicating that the temperatures of long-range magnetic ordering, T N , were below 0.45 K. Sr 2 Cu(PO 4 ) 2 and Ba 2 Cu(PO 4 ) 2 are an excellent physical realization of the S=1/2 linear chain Heisenberg antiferromagnet with k B T N /J 2 CuO 3 (k B T N /J∼0.25%) and γ-LiV 2 O 5 (k B T N /J 2 Cu(PO 4 ) 2 and Ba 2 Cu(PO 4 ) 2 were stable in air up to 1280 and 1150 K, respectively
Neutron and photon (light) scattering on solitons in the quasi-one-dimensional magnetics
Abdulloev, K O
1999-01-01
The general expression we have found earlier for the dynamics form-factor is used to analyse experiments on the neutron and photon (light) scattering by the gas of solitons in quasi-one-dimensional magnetics (Authors)
Spinons, Solitons, and Breathers in Quasi-One-Dimensional Magnets
Broholm, Collin
2006-03-01
By scattering neutrons from coordination polymer magnets, we contrast the effects of a uniform and a staggered magnetic field on the quantum critical state of a spin-1/2 chain. In a partially magnetized state of copper pyrazine dinitrate (CuPzN) we find bounded spectral continua indicating that neutrons scatter from spin-1/2 quasi-particle pairs [1]. The complex boundaries including an incommensurate soft spot result from a field induced shift in the Fermi points for these quasi-particles. The measurements indicate that the magnetized state of CuPzN remains quantum critical. Copper benzoate [2] and CuCl2^.2(dimethylsulfoxide) (CDC) [3] differ from CuPzN in that there are two spins per unit cell along the spin chain. Rather than continuous spectra, we find resolution limited gapped excitations when these materials are subject to high fields. So with two spins per unit cell, an applied field can drive the spin-1/2 chain away from criticality. The explanation for this effect was provided by Affleck and Oshikawa. The alternating coordination environment induces a transverse staggered field and spinon binding. The quantum sine-Gordon model is the relevant low energy field theory and it predicts soliton and breather excitations at specific energies and wave vectors that we compare to the experiments. We shall also compare a complete measurement of the dynamic spin correlation function for CDC in a field to exact diagonalization results for a spin-1/2 chain with a staggered and uniform magnetic field [4]. [1] M. B. Stone, D. H. Reich, C. Broholm, K. Lefmann, C. Rischel, C. P. Landee, and M. M. Turnbull, Phys. Rev. Lett. 91, 037205 (2003). [2] M. Kenzelmann, Y. Chien, C. Broholm, D. H. Reich, and Y. Qiu, Phys. Rev. Lett. 93, 017204 (2004). [3] D. C. Dender, P. R. Hammar, Daniel H. Reich, C. Broholm, and G. Aeppli, Phys. Rev. Lett. 79, 1750 (1997). [4] M. Kenzelmann, C. D. Batista, Y. Chen, C. Broholm, D. H. Reich, S. Park, and Y. Qiu, Phys. Rev. B 71, 094411 (2005).
Matsuda, M.; Onishi, H.; Okutani, A.; Ma, J.; Agrawal, H.; Hong, T.; Pajerowski, D. M.; Copley, J. R. D.; Okunishi, K.; Mori, M.; Kimura, S.; Hagiwara, M.
2017-07-01
BaCo2V2O8 consists of Co chains in which a Co2 + ion carries a fictitious spin 1/2 with Ising anisotropy. We performed elastic and inelastic neutron scattering experiments in BaCo2V2O8 in a magnetic field perpendicular to the c axis which is the chain direction. With applying magnetic field along the a axis at 3.5 K, the antiferromagnetic order with the easy axis along the c axis, observed in zero magnetic field, is completely suppressed at 8 T, while the magnetic field gradually induces an antiferromagnetic order with the spin component along the b axis. We also studied magnetic excitations as a function of transverse magnetic field. The lower boundary of the spinon excitations splits gradually with increasing magnetic field. The overall feature of the magnetic excitation spectra in the magnetic field is reproduced by the theoretical calculation based on the spin 1/2 X X Z antiferromagnetic chain model, which predicts that the dynamic magnetic structure factor of the spin component along the chain direction is enhanced and that along the field direction has clear incommensurate correlations.
Quasi-One-Dimensional Particle-in-Cell Simulation of Magnetic Nozzles
Ebersohn, Frans H.; Sheehan, J. P.; Gallimore, Alec D.; Shebalin, John V.
2015-01-01
A method for the quasi-one-dimensional simulation of magnetic nozzles is presented and simulations of a magnetic nozzle are performed. The effects of the density variation due to plasma expansion and the magnetic field forces on ion acceleration are investigated. Magnetic field forces acting on the electrons are found to be responsible for the formation of potential structures which accelerate ions. The effects of the plasma density variation alone are found to only weakly affect ion acceleration. Strongly diverging magnetic fields drive more rapid potential drops.
International Nuclear Information System (INIS)
Rogge, R.B.; Gaulin, B.D.; Harrison, A.
1992-01-01
Neutron scattering measurements have been performed on a single crystal sample of CsCo 0.83 Mg 0.17 Br 3 , a quasi-one-dimensional, Ising-like antiferromagnet. Residual three-dimensional interactions between the dilute magnetic chains precipitate a phase transition to long range order at T N ∼ 8.5 K, and short range correlations persist as high as 40 K. Relatively high energy inelastic scattering from both ''bulk'' spin wave modes and ''end'' modes is observed from the finite chains. The low energy inelastic spectrum is dominated by soliton scattering due to anti-phase domain walls propagating along the finite chains
Specific heat study of quasi-one-dimensional antiferromagnetic model for an organic polymer chain
International Nuclear Information System (INIS)
Qu Shaohua; Zhu Lin
2008-01-01
The specific heat of an infinite one-dimensional polymer chain bearing periodically arranged side radicals connected to the even sites is studied by means of quantum transfer-matrix method based on a Ising-Heisenberg model. In the absence of the exchange interactions between side radicals and the main chain, the curves of specific heat show a round peak due to the antiferromagnetic excitations for the all antiferromagnetic interactions along the polymer chain. Considering the exchange interactions between the side radicals and the main chain, the curves of the specific heat show double-peak structure for ferromagnetic interactions between the radicals and main chain, indicating that a competition between ferromagnetic and antiferromagnetic interactions and the possibility of the occurrence of the stable ferrimagnetic state along the polymer chain
Quasi-one-dimensional Heisenberg antiferromagnetic model for an organic polymeric chain
International Nuclear Information System (INIS)
Wu, F; Wang, W Z
2006-01-01
Using the exact diagonalization technique, we study the properties of the ground state of a spin-1/2 antiferromagnetic Heisenberg model for a zigzag polymer chain with side radicals connected to the even sites. We consider the nearest-neighbour exchange J and the next-nearest-neighbour exchange αJ along the main chain, and J 1 between the even site on the main chain and the radical site. For small α the ground state is ferrimagnetic. For α>α c1 , the ground state is a spiral phase, which is characterized by a peak of the static structure factor S(q) locating at an incommensurate value q max . For α>α c2 , the ground state is antiferromagnetic. With increasing J 1 , α c1 decreases while α c2 has a maximum at about J 1 = 0.5. For very small J 1 and α = 0.5, the spin configuration on the main chain is a product of nearest-neighbour singlets. In the antiferromagnetic phase, if J 1 is large enough the even site and the radical site form a singlet with exchange-decoupling from the odd site while the odd sites approximately form an antiferromagnetic chain
Observation of magnetoelastic effects in a quasi-one-dimensional spiral magnet
Wang, Chong; Yu, Daiwei; Liu, Xiaoqiang; Chen, Rongyan; Du, Xinyu; Hu, Biaoyan; Wang, Lichen; Iida, Kazuki; Kamazawa, Kazuya; Wakimoto, Shuichi; Feng, Ji; Wang, Nanlin; Li, Yuan
2017-08-01
We present a systematic study of spin and lattice dynamics in the quasi-one-dimensional spiral magnet CuBr2, using Raman scattering in conjunction with infrared and neutron spectroscopy. Along with the development of spin correlations upon cooling, we observe a rich set of broad Raman bands at energies that correspond to phonon-dispersion energies near the one-dimensional magnetic wave vector. The low-energy bands further exhibit a distinct intensity maximum at the spiral magnetic ordering temperature. We attribute these unusual observations to two possible underlying mechanisms: (1) formation of hybrid spin-lattice excitations and/or (2) "quadrumerization" of the lattice caused by spin-singlet entanglement in competition with the spiral magnetism.
Magnetic-field induced bistability in a quasi-one-dimensional semiconductor microcavity
International Nuclear Information System (INIS)
Zhang, Chuanyi; Zhang, Weifeng
2015-01-01
We theoretically study the magnetic-field induced bistability in a quasi-one-dimensional semiconductor microcavity. A critical magnetic field is obtained, and the bistability appears if a magnetic field is greater than the critical value. For a positive energy detuning of the pump from the bare exciton polaritons, one bistability loop first emerges, then it divides into two loops, and finally one of them vanishes with the increasing magnetic field. This phenomenon originates from the magnetic-field modulated interactions for opposite spins. In the variational process, there are two important effects: one is a logic gate with a small variation of the excitation laser, and the other is a spin texture like skyrmion and this texture is periodic if the energy detuning varies periodically in real space, which is useful for designing the spin-dependent optoelectronic devices. - Highlights: • We study the bistability induced by a magnetic field in a microcavity. • One bistability loop can divide into two, and then the two loops return to one. • A spin texture like skyrmion and logic gate arise in the variation of bistability loop
Quasi-one-dimensional magnetic behaviour of the Ising system CsFeCl3.2aq
Kopinga, K.; Steiner, M.; Jonge, de W.J.M.
1985-01-01
The magnetic behaviour of the quasi-one-dimensional system CsFeCl3.2aq(aq=H2O, D2O) has been investigated by heat capacity measurements, quasi-elastic neutron scattering and spin-cluster resonance. the experiments demonstrate that below 25K the compound is a very good realisation of an (S=1/2) Ising
Nocera, A.; Patel, N. D.; Fernandez-Baca, J.; Dagotto, E.; Alvarez, G.
2016-11-01
We study the effects of charge degrees of freedom on the spin excitation dynamics in quasi-one-dimensional magnetic materials. Using the density matrix renormalization group method, we calculate the dynamical spin structure factor of the Hubbard model at half electronic filling on a chain and on a ladder geometry, and compare the results with those obtained using the Heisenberg model, where charge degrees of freedom are considered frozen. For both chains and two-leg ladders, we find that the Hubbard model spectrum qualitatively resembles the Heisenberg spectrum—with low-energy peaks resembling spinonic excitations—already at intermediate on-site repulsion as small as U /t ˜2 -3 , although ratios of peak intensities at different momenta continue evolving with increasing U /t converging only slowly to the Heisenberg limit. We discuss the implications of these results for neutron scattering experiments and we propose criteria to establish the values of U /t of quasi-one-dimensional systems described by one-orbital Hubbard models from experimental information.
DEFF Research Database (Denmark)
Manuel, P.; Adroja, D. T.; Lindgård, Per-Anker
2011-01-01
The S = 3/2, quasi-one-dimensional (1D) zig-zag chain Heisenberg antiferromagnet Li3RuO4 has been investigated using heat capacity, inelastic neutron scattering, neutron diffraction, and μSR measurements on a powder sample. Our neutron diffraction and μSR studies confirm a long-range ordering of ...
Coupling of structure to magnetic and superconducting orders in quasi-one-dimensional K2Cr3As3
Taddei, K. M.; Zheng, Q.; Sefat, A. S.; de la Cruz, C.
2017-11-01
Quasi-one-dimensional A2Cr3As3 (with A =K , Cs, Rb) is an intriguing new family of superconductors which exhibit many similar features to the cuprate and iron-based unconventional superconductor families. Yet, in contrast to these systems, no charge or magnetic ordering has been observed which could provide the electronic correlations presumed necessary for an unconventional superconducting pairing mechanism—an absence which defies predictions of first-principles models. We report the results of neutron scattering experiments on polycrystalline K2Cr3As3 (Tc˜7 K ) which probed the low-temperature dynamics near Tc. Neutron diffraction data evidence a subtle response of the nuclear lattice to the onset of superconductivity while inelastic scattering reveals a highly dispersive column of intensity at the commensurate wave vector q =(00 1/2 ) which loses intensity beneath Tc—indicative of short-range magnetic fluctuations. Using linear spin-wave theory, we model the observed scattering and suggest a possible structure to the short-range magnetic order. These observations suggest that K2Cr3As3 is in close proximity to a magnetic instability and that the incipient magnetic order both couples strongly to the lattice and competes with superconductivity, in direct analogy with the iron-based superconductors.
NMR studies at high magnetic fields of LiVGe_2O_6, a quasi one-dimensional spin S=1 system
Vonlanthen, P.; Tanaka, K. B.; Clark, W. G.; Gavilano, J. L.; Ott, H. R.; Millet, P.; Mila, F.; Kuhns, P.; Reyes, A. P.; Moulton, W. G.
2001-03-01
We report ^7Li NMR studies of LiVGe_2O_6, a quasi one-dimensional spin S=1 system. Our measurements include NMR spectra, the spin-lattice relaxation rate, T_1-1, and the spin-spin relaxation rate, T_2-1, obtained at magnetic fields (B) of 9 and 23 T and temperatures (T) over the range 1.8 - 300 K. The 9 T NMR spectra show a continuous transfer of spectral weight from a paramagnetic phase to an antiferromagnetic one in a narrow temperature range of about 2 K around the transition temperature TN ≈ 25 K. Both phases coexist in this range. Below 10 K, well into the antiferromagnetic phase, the T_1-1 measurements are consistent with electron spin excitations across an energy gap (Δ) with Δ/k_B≈ 14 K at 9 T and 11 K at about 23 T; i.e., applying a large B slightly reduces Δ. Changing B from 9 to 23 T increases TN by 1 K. Thus, TN is influenced only marginally by B up to 23 Tesla. The UCLA part of the work was supported by NSF Grants DMR-9705369 and DMR-0072524.
Cabrera, I.; Thompson, J. D.; Coldea, R.; Prabhakaran, D.; Bewley, R. I.; Guidi, T.; Rodriguez-Rivera, J. A.; Stock, C.
2014-07-01
The quasi-one-dimensional (1D) Ising ferromagnet CoNb2O6 has recently been driven via applied transverse magnetic fields through a continuous quantum phase transition from spontaneous magnetic order to a quantum paramagnet, and dramatic changes were observed in the spin dynamics, characteristic of weakly perturbed 1D Ising quantum criticality. We report here extensive single-crystal inelastic neutron scattering measurements of the magnetic excitations throughout the three-dimensional (3D) Brillouin zone in the quantum paramagnetic phase just above the critical field to characterize the effects of the finite interchain couplings. In this phase, we observe that excitations have a sharp, resolution-limited line shape at low energies and over most of the dispersion bandwidth, as expected for spin-flip quasiparticles. We map the full bandwidth along the strongly dispersive chain direction and resolve clear modulations of the dispersions in the plane normal to the chains, characteristic of frustrated interchain couplings in an antiferromagnetic isosceles triangular lattice. The dispersions can be well parametrized using a linear spin-wave model that includes interchain couplings and further neighbor exchanges. The observed dispersion bandwidth along the chain direction is smaller than that predicted by a linear spin-wave model using exchange values determined at zero field, and this effect is attributed to quantum renormalization of the dispersion beyond the spin-wave approximation in fields slightly above the critical field, where quantum fluctuations are still significant.
NMR study of quasi-one-dimensional itinerant-electron magnets RMn{sub 4}Al{sub 8} (R=Y, Lu and Sc)
Energy Technology Data Exchange (ETDEWEB)
Muro, Y. [Graduate School of Material Science, University of Hyogo, Kamigori, Ako-gun, Hyogo 678-1297 (Japan)], E-mail: rk04j052@yahoo.co.jp; Nakamura, H.; Kohara, T. [Graduate School of Material Science, University of Hyogo, Kamigori, Ako-gun, Hyogo 678-1297 (Japan)
2008-04-01
{sup 55}Mn-NMR measurements, which revealed previously the presence of spin pseudogap in YMn{sub 4}Al{sub 8}, have been extended to LuMn{sub 4}Al{sub 8} and ScMn{sub 4}Al{sub 8}. Temperature (T) dependences of the Knight shift, K, and the nuclear spin-lattice relaxation rate, 1/T{sub 1}, are well explained by the same pseudogap model used to explain a broad maximum observed in the T-dependence of the susceptibility, indicating common nature in the spin excitation spectrum in the quasi-one-dimensional itinerant-electron compounds.
Quasi-one-dimensional intermittent flux behavior in superconducting films
Qviller, A. J.; Yurchenko, V. V.; Galperin, Y. M.; Vestgården, J. I.; Mozhaev, Peter; Hansen, Jørn Bindslev; Johansen, T. H.
2012-01-01
Intermittent filamentary dynamics of the vortex matter in superconductors is found in films of YBa_{2}Cu_{3}O_{7-δ} deposited on tilted substrates. Deposition of this material on such substrates creates parallel channels of easy flux penetration when a magnetic field is applied perpendicular to the film. As the applied field is gradually increased, magneto-optical imaging reveals that flux penetrates via numerous quasi-one-dimensional jumps. The distribution of flux avalanche sizes follows a ...
Quasi-One-Dimensional Intermittent Flux Behavior in Superconducting Films
Directory of Open Access Journals (Sweden)
A. J. Qviller
2012-01-01
Full Text Available Intermittent filamentary dynamics of the vortex matter in superconductors is found in films of YBa_{2}Cu_{3}O_{7-δ} deposited on tilted substrates. Deposition of this material on such substrates creates parallel channels of easy flux penetration when a magnetic field is applied perpendicular to the film. As the applied field is gradually increased, magneto-optical imaging reveals that flux penetrates via numerous quasi-one-dimensional jumps. The distribution of flux avalanche sizes follows a power law, and data collapse is obtained by finite-size scaling, with the depth of the flux front used as crossover length. The intermittent behavior shows no threshold value in the applied field, in contrast to conventional flux jumping. The results strongly suggest that the quasi-one-dimensional flux jumps are of a different nature than the thermomagnetic dendritic (branching avalanches that are commonly found in superconducting films.
International Nuclear Information System (INIS)
Shi, Y.G.; Guo, Y.F.; Yu, S.; Arai, M.; Belik, A.A.; Sato, A.; Yamaura, K.; Takayama-Muromachi, E.
2010-01-01
Na 2 OsO 4 crystals were grown by a NaCl flux method under high pressure. It crystallizes in the Ca 2 IrO 4 -type structure without having additional elements or metal vacancies, which are usually accommodated. It appears that Na 2 OsO 4 is a metal-stoichiometric Ca 2 IrO 4 -type compound never been synthesized to date. Na 2 OsO 4 has the octahedral environment of Os 6+ O 6 so that the electronic configuration is 5d 2 , suggesting the magnetic S=1 ground state. However, magnetization, electrical resistivity, and specific heat measurements indicated that the non-magnetic S=0 state is much likely for Na 2 OsO 4 than the S=1 state. Band structure calculations and the structure analysis found that the disagreement is probably due to the statically uniaxial compression of the OsO 6 octahedra, resulting in splitting of the t 2 g band. - Graphical abstract: Na 2 OsO 4 crystals were grown by a NaCl flux method under high pressure. It crystallizes in the Ca 2 IrO 4 -type structure comprising infinite Os 6+ O 6 octahedra (5d 2 ) chains. The crystal growth, the crystal structure, and the magnetic and electrical properties are reported.
Energy Technology Data Exchange (ETDEWEB)
Muro, Y. [Graduate School of Material Science, University of Hyogo, Kamigori, Ako-gun, Hyogo 678-1297 (Japan)]. E-mail: rk04j052@stkt.u-hyogo.ac.jp; Motoyama, G. [Graduate School of Material Science, University of Hyogo, Kamigori, Ako-gun, Hyogo 678-1297 (Japan); Nakamura, H. [Graduate School of Material Science, University of Hyogo, Kamigori, Ako-gun, Hyogo 678-1297 (Japan); Kohara, T. [Graduate School of Material Science, University of Hyogo, Kamigori, Ako-gun, Hyogo 678-1297 (Japan)
2006-05-01
Magnetovolume effects of 3d heavy-electron compounds with linear spin chains, (La{sub 1-x}Y{sub x})Mn{sub 4}Al{sub 8} with x=<0.15 and =1, have been investigated to get information on the ground state of LaMn{sub 4}Al{sub 8} and the nature of spin fluctuations in this system. The negative thermal expansion observed for LaMn{sub 4}Al{sub 8} is suppressed by the substitution of a small amount of Y for La. Together with the field-cooled effect in the susceptibility, the magnetovolume effect suggests the development of short-range magnetic correlation in LaMn{sub 4}Al{sub 8} at low temperatures.
The quantum flux in quasis one-dimensional conductors
International Nuclear Information System (INIS)
Ventura, J.
1989-01-01
A method is presented which quantizes electromagnetic fluxes directly in flux space. It is based on the commutation law [φ B , φ E ] = i, where φ B is the magnetic flux, and φ E the longitudinal electric flux of a quasi one-dimensional conductor. The relevance of such a method for the description of the quantized Hall plateaus is discussed. In a second step, the polarization electric flux is introduced, together with a method for quantization of hybrid variables formed with pure electromagnetic fluxes plus electronic variables. (author) [pt
Structural study of quasi-one-dimensional vanadium pyroxene LiVSi{sub 2}O{sub 6} single crystals
Energy Technology Data Exchange (ETDEWEB)
Ishii, Yuto [Department of Physics, Hokkaido University, Sapporo 060-0810 (Japan); Matsushita, Yoshitaka [National Institute for Materials Science, 1-1 Namiki, Tsukuba, Ibaraki 305-0044 (Japan); Oda, Migaku; Yoshida, Hiroyuki [Department of Physics, Hokkaido University, Sapporo 060-0810 (Japan)
2017-02-15
Single crystals of quasi-one-dimensional vanadium pyroxene LiVSi{sub 2}O{sub 6} were synthesized and the crystal structures at 293 K and 113 K were studied using X-ray diffraction experiments. We found a structural phase transition from the room-temperature crystal structure with space group C2/c to a low-temperature structure with space group P2{sub 1}/c, resulting from a rotational displacement of SiO{sub 4} tetrahedra. The temperature dependence of magnetic susceptibility shows a broad maximum around 116 K, suggesting an opening of the Haldane gap expected for one-dimensional antiferromagnets with S=1. However, an antiferromagnetic long-range order was developed below 24 K, probably caused by a weak inter-chain magnetic coupling in the compound. - Graphical abstract: Low temperature crystal structure of LiVSi{sub 2}O{sub 6} and an orbital arrangement within the V-O zig-zag chain along the c-axis. - Highlights: • A low temperature structure of LiVSi{sub 2}O{sub 6} was determined by single crystal X-ray diffraction measurements. • The origin of the structural transition is a rotational displacement of SiO{sub 4} tetrahedra. • The uniform orbital overlap in the V-O zigzag chain makes the system a quasi one-dimensional antiferromagnet.
Plasma properties of quasi-one-dimensional ring
Shmelev, G M
2001-01-01
The plasma properties of the quasi-one-dimensional ring in the threshold cases of low and high frequencies, corresponding to the plasma oscillations and dielectric relaxation are studied within the frames of the classical approach. The plasma oscillations spectrum and the electron dielectric relaxation frequency in the quasi-one-dimensional ring are calculated. The plasmons spectrum equidistance is identified. It is shown , that in contrast to the three-dimensional case there takes place the dielectric relaxation dispersion, wherefrom there follows the possibility of studying the carriers distribution in the quasi-one-dimensional rings through the method of the dielectric relaxation spectroscopy
Quasi-one-dimensional scattering in a discrete model
DEFF Research Database (Denmark)
Valiente, Manuel; Mølmer, Klaus
2011-01-01
We study quasi-one-dimensional scattering of one and two particles with short-range interactions on a discrete lattice model in two dimensions. One of the directions is tightly confined by an arbitrary trapping potential. We obtain the collisional properties of these systems both at finite and zero...
Current-Voltage Characteristics of Quasi-One-Dimensional Superconductors
DEFF Research Database (Denmark)
Vodolazov, D.Y.; Peeters, F.M.; Piraux, L.
2003-01-01
The current-voltage (I-V) characteristics of quasi-one-dimensional superconductors were discussed. The I-V characteristics exhibited an unusual S behavior. The dynamics of superconducting condensate and the existence of two different critical currents resulted in such an unusual behavior....
Energy Technology Data Exchange (ETDEWEB)
Azuma, M.; Hiroi, Z.; Takano, M. [Kyoto Univ. (Japan)] [and others
1994-12-31
SrCu{sub 2}O{sub 3} and Sr{sub 2}Cu{sub 3}O{sub 5} containing two-leg and three-leg S=1/2 ladders made of antiferromagnetic Cu-O-Cu linear bonds, respectively, were synthesized at high pressure, and their crystallographic and magnetic properties were investigated. Both susceptibility and T{sub 1} data of NMR revealed the existence of a large spin gap only for SrCu{sub 2}O{sub 3}. Superconductivity, which had been predicted theoretically for carrier-doped SrCu{sub 2}O{sub 3} could not be realized although partial substitution of La{sup 3+} for Sr{sup 2+} seemed to be carried out successfully. Electron carriers injected seems to remain localized.
Yamauchi, Ichihiro; Itoh, Masayuki; Yamauchi, Touru; Yamaura, Jun-Ichi; Ueda, Yutaka
2017-11-01
51V NMR measurements have been conducted on a single crystal of the quasi-one-dimensional conductor β -Li0.33V2O5 which undergoes a metal-insulator (MI) transition at TMI˜170 K. In the metallic phase, we obtain 51V Knight shift and electric field gradient tensors. From the analysis of the 51V Knight shifts, we find that the charge disproportionation appears even in the metallic state and the electronic structure is represented within a model of weakly coupled ladders containing two types of ladders with distinct carrier densities. Based on the 51V nuclear spin-lattice relaxation rate, we discuss the spin dynamics within the one-dimensional electron gas model. From the analysis of several nonmagnetic V5 + spectra observed in the insulating phase, we propose a possible charge-order pattern which has a superlattice modulation larger than those in other family members of β -A0.33V2O5 (A =Na and Ag). Finally, we discuss the A -ion dependence of the electronic structure, the charge disproportionation, and the charge order in β -A0.33V2O5 .
Energy Technology Data Exchange (ETDEWEB)
Petukhov, B. V., E-mail: petukhov@ns.crys.ras.ru [Russian Academy of Sciences, Shubnikov Institute of Crystallography, Federal Scientific Research Centre “Crystallography and Photonics,” (Russian Federation)
2017-01-15
The state switching in an extended quasi-one-dimensional material is modeled by the stochastic formation of local new-state nuclei and their subsequent growth along the system axis. An analytical approach is developed to describe the influence of defects, dividing a sample into an ensemble of finite-length segments, on its state switching kinetics. As applied to magnetic systems, the method makes it possible to calculate magnetization curves for different defect concentrations and parameters of material.
Quasi-one-dimensional metals on semiconductor surfaces with defects
International Nuclear Information System (INIS)
Hasegawa, Shuji
2010-01-01
Several examples are known in which massive arrays of metal atomic chains are formed on semiconductor surfaces that show quasi-one-dimensional metallic electronic structures. In this review, Au chains on Si(557) and Si(553) surfaces, and In chains on Si(111) surfaces, are introduced and discussed with regard to the physical properties determined by experimental data from scanning tunneling microscopy (STM), angle-resolved photoemission spectroscopy (ARPES) and electrical conductivity measurements. They show quasi-one-dimensional Fermi surfaces and parabolic band dispersion along the chains. All of them are known from STM and ARPES to exhibit metal-insulator transitions by cooling and charge-density-wave formation due to Peierls instability of the metallic chains. The electrical conductivity, however, reveals the metal-insulator transition only on the less-defective surfaces (Si(553)-Au and Si(111)-In), but not on a more-defective surface (Si(557)-Au). The latter shows an insulating character over the whole temperature range. Compared with the electronic structure (Fermi surfaces and band dispersions), the transport property is more sensitive to the defects. With an increase in defect density, the conductivity only along the metal atomic chains was significantly reduced, showing that atomic-scale point defects decisively interrupt the electrical transport along the atomic chains and hide the intrinsic property of transport in quasi-one-dimensional systems.
Quasi-one-dimensional Hall physics in the Harper–Hofstadter–Mott model
Kozarski, Filip; Hügel, Dario; Pollet, Lode
2018-04-01
We study the ground-state phase diagram of the strongly interacting Harper–Hofstadter–Mott model at quarter flux on a quasi-one-dimensional lattice consisting of a single magnetic flux quantum in y-direction. In addition to superfluid phases with various density patterns, the ground-state phase diagram features quasi-one-dimensional analogs of fractional quantum Hall phases at fillings ν = 1/2 and 3/2, where the latter is only found thanks to the hopping anisotropy and the quasi-one-dimensional geometry. At integer fillings—where in the full two-dimensional system the ground-state is expected to be gapless—we observe gapped non-degenerate ground-states: at ν = 1 it shows an odd ‘fermionic’ Hall conductance, while the Hall response at ν = 2 consists of the transverse transport of a single particle–hole pair, resulting in a net zero Hall conductance. The results are obtained by exact diagonalization and in the reciprocal mean-field approximation.
Effects of weak localization in quasi-one-dimensional electronic system over liquid helium
Kovdrya, Y Z; Gladchenko, S P
2001-01-01
One measured rho sub x sub x magnetoresistance of a quasi-one-dimensional electronic system over liquid helium within gas scattering range (1.3-2.0 K temperature range). It is shown that with increase of magnetic field the magnetoresistance is reduced at first and them upon passing over minimum it begins to increase from rho sub x sub x approx B sup 2 law. One anticipated that the negative magnetoresistance detected in the course of experiments resulted from the effects of weak localization. The experiment results are in qualitative conformity with the theoretical model describing processes of weak localization in single-dimensional nondegenerate electronic systems
International Nuclear Information System (INIS)
Papp, E.; Micu, C.; Racolta, D.
2013-01-01
In this paper one deals with the theoretical derivation of energy bands and of related wavefunctions characterizing quasi 1D semiconductor heterostructures, such as InAs quantum wire models. Such models get characterized this time by equal coupling strength superpositions of Rashba and Dresselhaus spin-orbit interactions of dimensionless magnitude a under the influence of in-plane magnetic fields of magnitude B. We found that the orientations of the field can be selected by virtue of symmetry requirements. For this purpose one resorts to spin conservations, but alternative conditions providing sensible simplifications of the energy-band formula can be reasonably accounted for. Besides the wavenumber k relying on the 1D electron, one deals with the spin-like s=±1 factors in the front of the square root term of the energy. Having obtained the spinorial wavefunction, opens the way to the derivation of spin precession effects. For this purpose one resorts to the projections of the wavenumber operator on complementary spin states. Such projections are responsible for related displacements proceeding along the Ox-axis. This results in a 2D rotation matrix providing both the precession angle as well as the precession axis
Shell-crossing in quasi-one-dimensional flow
Rampf, Cornelius; Frisch, Uriel
2017-10-01
Blow-up of solutions for the cosmological fluid equations, often dubbed shell-crossing or orbit crossing, denotes the breakdown of the single-stream regime of the cold-dark-matter fluid. At this instant, the velocity becomes multi-valued and the density singular. Shell-crossing is well understood in one dimension (1D), but not in higher dimensions. This paper is about quasi-one-dimensional (Q1D) flow that depends on all three coordinates but differs only slightly from a strictly 1D flow, thereby allowing a perturbative treatment of shell-crossing using the Euler-Poisson equations written in Lagrangian coordinates. The signature of shell-crossing is then just the vanishing of the Jacobian of the Lagrangian map, a regular perturbation problem. In essence, the problem of the first shell-crossing, which is highly singular in Eulerian coordinates, has been desingularized by switching to Lagrangian coordinates, and can then be handled by perturbation theory. Here, all-order recursion relations are obtained for the time-Taylor coefficients of the displacement field, and it is shown that the Taylor series has an infinite radius of convergence. This allows the determination of the time and location of the first shell-crossing, which is generically shown to be taking place earlier than for the unperturbed 1D flow. The time variable used for these statements is not the cosmic time t but the linear growth time τ ˜ t2/3. For simplicity, calculations are restricted to an Einstein-de Sitter universe in the Newtonian approximation, and tailored initial data are used. However it is straightforward to relax these limitations, if needed.
Magnetic field effects of tow-leg Heisenberg antiferromagnetic ladders: Thermodynamic properties
International Nuclear Information System (INIS)
Wang Xiaoqun; Yu Lu
2000-05-01
Using the recently developed transfer-matrix renormalization group method, we have studied the thermodynamic properties of two-leg antiferromagnetic ladders in the magnetic field. Based on different behavior of magnetization, we found disordered spin liquid, Luttinger liquid, spin-polarized phases and a classical regime depending on magnetic field and temperature. Our calculations in Luttinger liquid regime suggest that both the divergence of the NMR relaxation rate and the anomalous specific heat behavior observed on Cu 2 (C 5 H 12 N 2 ) 2 Cl 4 are due to quasi-one-dimensional effect rather than three-dimensional ordering. (author)
Magnetotransport in a quasi-one-dimensional electron system over superfluid helium
Nikolaenko, V A; Gladchenko, S P
2002-01-01
Magnetotransport in a nondegenerate quasi-one-dimensional electron system (Q1D) over superfluid helium is investigated experimentally. The experiments were carried out at perpendicular magnetic fields, B 0.9 K) and the electron-ripplon scattering (T 1(here omega sub c is the cyclotron frequency and t is the relaxation time of the electron system) agree qualitatively with the self-consistent Born approximation theory for a 2D electron system over helium. It is supposed that the quantitative discrepancies in the experimental and theoretical data are connected with different peculiar features of the investigated and analyzed electron systems. The experimental data on electron mobility at low temperatures and small magnetic fields coincide with the theoretical calculation made for the Q1D system. The negative magnetoresistance of the channels observed both in the electron-gas scattering and electron-ripplon scattering regions is supposed to be due to weak localization of carriers in the investigated electron syst...
Quantum Fluctuations in Quasi-One-Dimensional Dipolar Bose-Einstein Condensates.
Edler, D; Mishra, C; Wächtler, F; Nath, R; Sinha, S; Santos, L
2017-08-04
Recent experiments have revealed that beyond-mean-field corrections are much more relevant in weakly interacting dipolar condensates than in their nondipolar counterparts. We show that in quasi-one-dimensional geometries quantum corrections in dipolar and nondipolar condensates are strikingly different due to the peculiar momentum dependence of the dipolar interactions. The energy correction of the condensate presents not only a modified density dependence, but it may even change from attractive to repulsive at a critical density due to the surprising role played by the transversal directions. The anomalous quantum correction translates into a strongly modified physics for quantum-stabilized droplets and dipolar solitons. Moreover, and for similar reasons, quantum corrections of three-body correlations, and hence of three-body losses, are strongly modified by the dipolar interactions. This intriguing physics can be readily probed in current experiments with magnetic atoms.
Quasi-one-dimensional intermittent flux behavior in superconducting films
DEFF Research Database (Denmark)
Qviller, A. J.; Yurchenko, V. V.; Galperin, Y. M.
2012-01-01
Intermittent filamentary dynamics of the vortex matter in superconductors is found in films of YBa2Cu3O7-δ deposited on tilted substrates. Deposition of this material on such substrates creates parallel channels of easy flux penetration when a magnetic field is applied perpendicular to the film. ...
Prediction of inorganic superconductors with quasi-one-dimensional crystal structure
International Nuclear Information System (INIS)
Volkova, L M; Marinin, D V
2013-01-01
Models of superconductors having a quasi-one-dimensional crystal structure based on the convoluted into a tube Ginzburg sandwich, which comprises a layered dielectric–metal–dielectric structure, have been suggested. The critical crystal chemistry parameters of the Ginzburg sandwich determining the possibility of the emergence of superconductivity and the T c value in layered high-T c cuprates, which could have the same functions in quasi-one-dimensional fragments (sandwich-type tubes), have been examined. The crystal structures of known low-temperature superconductors, in which one can mark out similar quasi-one-dimensional fragments, have been analyzed. Five compounds with quasi-one-dimensional structures, which can be considered as potential parents of new superconductor families, possibly with high transition temperatures, have been suggested. The methods of doping and modification of these compounds are provided. (paper)
Magnetotransport in a quasi-one-dimensional electron system over superfluid helium
International Nuclear Information System (INIS)
Nikolaenko, V.A.; Kovdrya, Yu.Z.; Gladchenko, S.P.
2002-01-01
Magnetotransport in a nondegenerate quasi-one-dimensional electron system (Q1D) over superfluid helium is investigated experimentally. The experiments were carried out at perpendicular magnetic fields, B xx of the conducting channels mainly grows with increasing B for both the electron-gas atom scattering (T > 0.9 K) and the electron-ripplon scattering (T c τ>1(here ω c is the cyclotron frequency and t is the relaxation time of the electron system) agree qualitatively with the self-consistent Born approximation theory for a 2D electron system over helium. It is supposed that the quantitative discrepancies in the experimental and theoretical data are connected with different peculiar features of the investigated and analyzed electron systems. The experimental data on electron mobility at low temperatures and small magnetic fields coincide with the theoretical calculation made for the Q1D system. The negative magnetoresistance of the channels observed both in the electron-gas scattering and electron-ripplon scattering regions is supposed to be due to weak localization of carriers in the investigated electron system
Metal-Insulator Phase Transition in Quasi-One-Dimensional VO2 Structures
Directory of Open Access Journals (Sweden)
Woong-Ki Hong
2015-01-01
Full Text Available The metal-insulator transition (MIT in strongly correlated oxides has attracted considerable attention from both theoretical and experimental researchers. Among the strongly correlated oxides, vanadium dioxide (VO2 has been extensively studied in the last decade because of a sharp, reversible change in its optical, electrical, and magnetic properties at approximately 341 K, which would be possible and promising to develop functional devices with advanced technology by utilizing MITs. However, taking the step towards successful commercialization requires the comprehensive understanding of MIT mechanisms, enabling us to manipulate the nature of transitions. In this regard, recently, quasi-one-dimensional (quasi-1D VO2 structures have been intensively investigated due to their attractive geometry and unique physical properties to observe new aspects of transitions compared with their bulk counterparts. Thus, in this review, we will address recent research progress in the development of various approaches for the modification of MITs in quasi-1D VO2 structures. Furthermore, we will review recent studies on realizing novel functional devices based on quasi-1D VO2 structures for a wide range of applications, such as a gas sensor, a flexible strain sensor, an electrical switch, a thermal memory, and a nonvolatile electrical memory with multiple resistance.
Magnetic Properties of the S=2 Heisenberg Antiferromagnetic Chain Compound MnCl3(bpy)
International Nuclear Information System (INIS)
Hagiwara, M; Idutsu, Y; Honda, Z; Yamamoto, S
2012-01-01
We report the results of magnetic susceptibilities at temperatures between 2 and 300 K, and magnetization in magnetic fields of up to 52 T on polycrystalline samples of MnCl 3 (bpy) (bpy=2, 2'-bipyridine) and the comparison with numerical calculations. This compound is one of the rare examples of the spin 2 quasi-one-dimensional Heisenberg antiferromagnet, and the magnetic properties of tiny single crystal samples were reported previously. The temperature dependence of magnetic susceptibility and the magnetization curve after subtracting the contribution of magnetic impurity are well fitted to those calculated by a quantum Monte Carlo method with the intrachain exchange constant J/k B =31.2 K and the g-value g=2.02 which are comparable to reported values (J/k B =34.8±1.6 K and g=2.04±0.04).
Optimally localized Wannier functions for quasi one-dimensional nonperiodic insulators
DEFF Research Database (Denmark)
Cornean, Horia; Nenciu, A.; Nenciu, Gheorghe
2008-01-01
It is proved that for general, not necessarily periodic, quasi one-dimensional systems the band position operator corresponding to an isolated part of the energy spectrum has discrete spectrum and its eigenfunctions have the same spatial localization as the corresponding spectral projection....... As a consequence, an eigenbasis of the band position operator provides a basis of optimally localized (generalized) Wannier functions for quasi one-dimensional systems, and this proves the strong Marzari-Vanderbilt conjecture. If the system has some translation symmetries (e.g. usual translations, screw...
Optimally localized Wannier functions for quasi one-dimensional nonperiodic insulators
DEFF Research Database (Denmark)
Cornean, Horia; Nenciu, A.; Nenciu, Gheorghe
It is proved that for general, not necessarily periodic quasi one dimensional systems, the band position operator corresponding to an isolated part of the energy spectrum has discrete spectrum and its eigenfunctions have the same spatial localization as the corresponding spectral projection....... As a consequence, an eigenbasis of the band position operator provides a basis of optimally localized (generalized) Wannier functions for quasi one dimensional systems. If the system has some translation symmetries (e.g. usual translations, screw transformations), they are "inherited" bythe Wannier basis....
Spin-zero sound in one- and quasi-one-dimensional 3He
International Nuclear Information System (INIS)
Hernandez, E.S.
2002-01-01
The zero sound spectrum of fluid 3 He confined to a cylindrical shell is examined for configurations characterizing strictly one-dimensional and quasi-one-dimensional regimes. It is shown that the restricted dimensionality makes room to the possibility of spin-zero sound for the attractive particle-hole interaction of liquid helium. This fact can be related to the suppression of phase instabilities and thermodynamic phase transitions in one dimension
Electronic structure of the quasi-one-dimensional organic conductor TTF-TCNQ
DEFF Research Database (Denmark)
Sing, M.; Schwingenschlögl, U.; Claessen, R.
2003-01-01
We study the electronic structure of the quasi-one-dimensional organic conductor TTF-TCNQ by means of density-functional band theory, Hubbard model calculations, and angle-resolved photoelectron spectroscopy (ARPES). The experimental spectra reveal significant quantitative and qualitative......-dimensional Hubbard model for the low-energy spectral behavior is attributed to interchain coupling and the additional effect of electron-phonon interaction....
Thermal conductivity of a quantum spin-1/2 antiferromagnetic chain with magnetic impurities
International Nuclear Information System (INIS)
Zviagin, A.A.
2008-01-01
We present an exact theory that describes how magnetic impurities change the behavior of the thermal conductivity for the integrable Heisenberg antiferromagnetic quantum spin-1/2 chain. Single magnetic impurities and a large concentration of impurities with similar values of the couplings to the host chain (a weak disorder) do not change the linear-in-temperature low-T behavior of the thermal conductivity: Only the slope of that behavior becomes smaller, compared to the homogeneous case. The strong disorder in the distribution of the impurity-host couplings produces more rapid temperature growth of the thermal conductivity, compared to the linear-in-T dependence of the homogeneous chain and the chain with weak disorder. Recent experiments on the thermal conductivity in inhomogeneous quasi-one-dimensional quantum spin systems manifest qualitative agreement with our results
How to manipulate magnetic states of antiferromagnets
Song, Cheng; You, Yunfeng; Chen, Xianzhe; Zhou, Xiaofeng; Wang, Yuyan; Pan, Feng
2018-03-01
Antiferromagnetic materials, which have drawn considerable attention recently, have fascinating features: they are robust against perturbation, produce no stray fields, and exhibit ultrafast dynamics. Discerning how to efficiently manipulate the magnetic state of an antiferromagnet is key to the development of antiferromagnetic spintronics. In this review, we introduce four main methods (magnetic, strain, electrical, and optical) to mediate the magnetic states and elaborate on intrinsic origins of different antiferromagnetic materials. Magnetic control includes a strong magnetic field, exchange bias, and field cooling, which are traditional and basic. Strain control involves the magnetic anisotropy effect or metamagnetic transition. Electrical control can be divided into two parts, electric field and electric current, both of which are convenient for practical applications. Optical control includes thermal and electronic excitation, an inertia-driven mechanism, and terahertz laser control, with the potential for ultrafast antiferromagnetic manipulation. This review sheds light on effective usage of antiferromagnets and provides a new perspective on antiferromagnetic spintronics.
Specific heat of S=1 quasi-1D antiferromagnet NDMAP in magnetic fields
International Nuclear Information System (INIS)
Tsujii, H.; Honda, Z.; Andraka, B.; Katsumata, K.; Takano, Y.
2003-01-01
NDMAP, Ni(C 5 H 14 N 2 ) 2 N 3 (PF 6 ), is a quasi-one-dimensional S=1 Heisenberg antiferromagnet with Haldane-gap energies of 22 and 5.5 K for excitations polarized parallel and perpendicular to the chain c-axis, respectively. We have extended the specific-heat measurements by Honda et al. in this compound to 150 mK in temperature and 18 T in magnetic field, employing a novel relaxation calorimeter. The experiment provides an accurate determination of the exponent for the transition line for the field-assisted ordered phase. In addition, a new feature has been found in the phase diagram at around 14 T
A quasi-one-dimensional model for the Giacobini-Zinner plasma tail
International Nuclear Information System (INIS)
Malara, F.; Einaudi, G.; Mangeney, A.
1989-01-01
An assumption of quasi-one-dimensionality is used to derive a simple set of equations describing the comet Giacobini-Zinner tail configuration. The MHD equations are expanded in terms of a parameter representing the ratio of the length scale in the direction perpendicular to the neutral sheet over the length scale in the direction parallel to the tail. It is shown that in this way it is possible to obtain much information on the structure of the tail and to fit reasonably well the observations made by the ICE spacecraft
Electron energy-loss spectroscopy of quasi-one-dimensional cuprates and vanadates
International Nuclear Information System (INIS)
Atzkern, S.
2001-01-01
In a combination of experimental and theoretical methods in this thesis the electronic structures of quasi-one-dimensional cuprates and vanadates were studied. For this the momentum-dependent loss function was measured by means of the electron energy-loss spectroscopy in transmission on monocrystals of Li 2 CuO 2 , CuGeO 3 , V 2 O 5 and α'-NaVO 5 . The comparison of the experimental data with results from band-structure and cluster calculations allowed conclusions on the mobility and correlations of the electrons in these systems
Quasi-one-dimensional electron transport over the surface of a liquid-helium film
International Nuclear Information System (INIS)
Sokolov, Sviatoslav; Studart, Nelson
2003-01-01
Quasi-one-dimensional mobility of surface electrons over a liquid-helium suspended film is studied for a conducting channel. The electron mobility is calculated taking into account the electron scattering by helium atoms in the vapor phase, ripplons, and surface defects of the film substrate both in one-electron regime and in the so-called complete-control limit where the influence of inter-electron collisions on the electron distribution function is taken into account. It is shown that the mobility for low temperatures is dominated by the surface-defect scattering and its temperature dependence is essentially different from that of the electron-ripplon scattering
Electronic structure and transport properties of quasi-one-dimensional carbon nanomaterials
Directory of Open Access Journals (Sweden)
Y. N. Wu
2017-09-01
Full Text Available Based on the density functional theory combined with the nonequilibrium Green’s function, the influence of the wrinkle on the electronic structures and transport properties of quasi-one-dimensional carbon nanomaterials have been investigated, in which the wrinkled armchair graphene nanoribbons (wAGNRs and the composite of AGNRs and single walled carbon nanotubes (SWCNTs were considered with different connection of ripples. The wrinkle adjusts the electronic structures and transport properties of AGNRs. With the change of the strain, the wAGNRs for three width families reveal different electrical behavior. The band gap of AGNR(6 increases in the presence of the wrinkle, which is opposite to that of AGNR(5 and AGNR(7. The transport of AGNRs with the widths 6 or 7 has been modified by the wrinkle, especially by the number of isolated ripples, but it is insensitive to the strain. The nanojunctions constructed by AGNRs and SWCNTs can form the quantum wells, and some specific states are confined in wAGNRs. Although these nanojunctions exhibit the metallic, they have poor conductance due to the wrinkle. The filling of C20 into SWCNT has less influence on the electronic structure and transport of the junctions. The width and connection type of ripples have greatly influenced on the electronic structures and transport properties of quasi-one-dimensional nanomaterials.
The electronic structure of quasi-one-dimensional disordered systems with parallel multi-chains
International Nuclear Information System (INIS)
Liu Xiaoliang; Xu Hui; Deng Chaosheng; Ma Songshan
2006-01-01
For the quasi-one-dimensional disordered systems with parallel multi-chains, taking a special method to code the sites and just considering the nearest-neighbor hopping integral, we write the systems' Hamiltonians as precisely symmetric matrixes, which can be transformed into three diagonally symmetric matrixes by using the Householder transformation. The densities of states, the localization lengths and the conductance of the systems are calculated numerically using the minus eigenvalue theory and the transfer matrix method. From the results of quasi-one-dimensional disordered systems with varied chains, we find, the energy band of the systems extends slightly, the energy gaps are observed and the distribution of the density of states changes obviously with the increase of the dimensionality. Especially, for the systems with four, five or six chains, at the energy band center, there exist extended states whose localization lengths are greater than the size of the systems, accordingly, there having great conductance. With the increasing of the number of the chains, the correlated ranges expand and the systems present the similar behavior to that with off-diagonal long-range correlation
Electronic structure and transport properties of quasi-one-dimensional carbon nanomaterials
Wu, Y. N.; Cheng, P.; Wu, M. J.; Zhu, H.; Xiang, Q.; Ni, J.
2017-09-01
Based on the density functional theory combined with the nonequilibrium Green's function, the influence of the wrinkle on the electronic structures and transport properties of quasi-one-dimensional carbon nanomaterials have been investigated, in which the wrinkled armchair graphene nanoribbons (wAGNRs) and the composite of AGNRs and single walled carbon nanotubes (SWCNTs) were considered with different connection of ripples. The wrinkle adjusts the electronic structures and transport properties of AGNRs. With the change of the strain, the wAGNRs for three width families reveal different electrical behavior. The band gap of AGNR(6) increases in the presence of the wrinkle, which is opposite to that of AGNR(5) and AGNR(7). The transport of AGNRs with the widths 6 or 7 has been modified by the wrinkle, especially by the number of isolated ripples, but it is insensitive to the strain. The nanojunctions constructed by AGNRs and SWCNTs can form the quantum wells, and some specific states are confined in wAGNRs. Although these nanojunctions exhibit the metallic, they have poor conductance due to the wrinkle. The filling of C20 into SWCNT has less influence on the electronic structure and transport of the junctions. The width and connection type of ripples have greatly influenced on the electronic structures and transport properties of quasi-one-dimensional nanomaterials.
Defects in quasi-one dimensional oxide conductors: K0.3MoO3
International Nuclear Information System (INIS)
Smith, K.E.; Breuer, K.; Goldberg, D.; Greenblatt, M.; McCarroll, W.; Hulbert, S.L.
1995-01-01
The electronic structure of the prototypical quasi-one dimensional (ID) conductor K 0.3 MoO 3 has been studied using high resolution photoemission spectroscopy. In particular, the electronic structure of defects was investigated in order to understand the mechanism for charge density wave pinning and destruction of the Peierls transition. Defects were found to radically alter the electronic structure close to the Fermi level (E F ), thus strongly modifying the structure of the Fermi surface. While a low emission intensity at E F has been interpreted as evidence for a Luttinger liquid ground state in a 1D metal, the authors show that non-stoichiometric surfaces lead to similar effects. The nature of the ground state is discussed in the context of these results
Sensitivity analysis explains quasi-one-dimensional current transport in two-dimensional materials
DEFF Research Database (Denmark)
Boll, Mads; Lotz, Mikkel Rønne; Hansen, Ole
2014-01-01
We demonstrate that the quasi-one-dimensional (1D) current transport, experimentally observed in graphene as measured by a collinear four-point probe in two electrode configurations A and B, can be interpreted using the sensitivity functions of the two electrode configurations (configurations...... A and B represents different pairs of electrodes chosen for current sources and potential measurements). The measured sheet resistance in a four-point probe measurement is averaged over an area determined by the sensitivity function. For a two-dimensional conductor, the sensitivity functions for electrode...... configurations A and B are different. But when the current is forced to flow through a percolation network, e.g., graphene with high density of extended defects, the two sensitivity functions become identical. This is equivalent to a four-point measurement on a line resistor, hence quasi-1D transport...
Lattice relaxation theory of localized excitations in quasi-one-dimensional systems
International Nuclear Information System (INIS)
Wang Chuilin; Su Zhaobin; Yu Lu.
1993-04-01
The lattice relaxation theory developed earlier by Su and Yu for solitons and polarons in conducting polymers is applied to systems with both electron-phonon and electron-electron interactions, described by a single band Peierls-Hubbard model. The localized excitations in the competing bond-order-wave (BOW), charge-density-wave (CDW) and spin-density-wave (SDW) systems show interesting new features in their dynamics. In particular, a non-monotonic dependence of the relaxation rate on the coupling strength is predicted from the theory. The possible connection of this effect with photo-luminescence experiments is discussed. Similar phenomena may occur in other quasi-one-dimensional systems as well. (author). 21 refs, 4 figs
Topological superconductor in quasi-one-dimensional Tl2 -xMo6Se6
Huang, Shin-Ming; Hsu, Chuang-Han; Xu, Su-Yang; Lee, Chi-Cheng; Shiau, Shiue-Yuan; Lin, Hsin; Bansil, Arun
2018-01-01
We propose that the quasi-one-dimensional molybdenum selenide compound Tl2 -xMo6Se6 is a time-reversal-invariant topological superconductor induced by intersublattice pairing, even in the absence of spin-orbit coupling (SOC). No noticeable change in superconductivity is observed in Tl-deficient (0 ≤x ≤0.1 ) compounds. At weak SOC, the superconductor prefers the triplet d vector lying perpendicular to the chain direction and two-dimensional E2 u symmetry, which is driven to a nematic order by spontaneous rotation symmetry breaking. The locking energy of the d vector is estimated to be weak and hence the proof of its direction would rely on tunneling or phase-sensitive measurements.
Solitons and polarons in quasi-one dimensional conducting polymers and related materials
International Nuclear Information System (INIS)
Campbell, D.K.
1983-01-01
In recent years it has become increasingly appreciated that fundamentally nonlinear excitations - solitons - play an essential role in an incredible variety of natural systems. These solitons, which frequently exhibit remarkable stability under interactions and perturbations, often dominate the transport, response, or structural properties of the systems in which they occur. In this article, we present an introduction to the solitons that occur in quasi-one-dimensional conducting polymers (synmetals) and related systems. The relevance of this subject to molecular electronic devices is twofold. First, many of these materials have molecular structures similar to possible prototype molecular switches. Second, to understand in detail how a molecular electronic device could work, it is essential to have a broad perspective on the nature of possible excitations in a variety of natural and synthetic molecular materials. 51 references
Polyacene and a new class of quasi-one-dimensional conductors
International Nuclear Information System (INIS)
Kivelson, S.; Chapman, O.L.
1983-01-01
Most one-dimensional conductors are quite similar since the Fermi surface is a point and the electron energy dispersion relation near the Fermi surface is linear. It is pointed out that in polyacene the Fermi surface lies at the edge of the Brillouin zone, but that an accidental degeneracy between the valence and conduction bands makes it metallic nonetheless. The dispersion relation is therefore quadratic, and the density of states diverges at the Fermi surface. Thus, polyacene [(C 4 H 2 )/sub n/] and its possible derivatives represent a conceptually new class of quasi-one-dimensional conductors. Moreover, we find that this class of materials has the possibility of possessing interesting condensed phases including high-temperature superconductivity and ferromagnetism
Ordering kinetics in quasi-one-dimensional Ising-like systems
International Nuclear Information System (INIS)
Mueller, M.; Paul, W.
1993-01-01
Results are presented of a Monte Carlo simulation of the kinetics of ordering in the two-dimensional nearest-neighbor Ising model in an L x M geometry with two free boundaries of length M much-gt L. This model can be viewed as representing an adsorbant on a stepped surface with mean terrace width L. The authors follow the ordering kinetics after quenches to temperatures 0.25 ≤T/T c ≤1 starting from a random initial configuration at a coverage of Θ=0.5 in the corresponding lattice gas picture. The systems evolve in time according to a Glauber kinetics with nonconserved order parameter. The equilibrium structure is given by a one-dimensional sequence of ordered domains. The ordering process evolves from a short initial two-dimensional ordering process through a crossover region to a quasi-one-dimensional behavior. The whole process is diffusive (inverse half-width of the structure factor peak 1/Δq parallel ∝ √t), in contrast to a model proposed by Kawasaki et al., where an intermediate logarithmic growth law is expected. All results are completely describable in the picture of an annihilating random walk (ARW) of domain walls. 36 refs., 16 figs
Unconventional Andreev reflection on the quasi-one-dimensional superconductor Nb2PdxSe5
Directory of Open Access Journals (Sweden)
Yeping Jiang
2016-04-01
Full Text Available We have carried out Andreev reflection measurements on point contact junctions between normal metal and single crystals of the quasi-one-dimensional (Q1D superconductor Nb2PdxSe5 (Tc ∼ 5.5 K. The contacts of the junctions were made on either self-cleaved surfaces or crystal edges so that the current flow directions in the two types of junctions are different, and the measurements provide a directional probe for the order parameter of the superconductor. Junctions made in both configurations show typical resistances of ∼20-30 Ohms, and a clear double-gap Andreev reflection feature was consistently observed at low temperatures. Quantitative analysis of the conductance spectrum based on a modified Blonder-Tinkham-Klapwijk (BTK model suggests that the amplitudes of two order parameters may have angular dependence in the a-c plane. Moreover, the gap to transition temperature ratio (Δ/TC for the larger gap is substantially higher than the BCS ratio expected for phonon-mediated s-wave superconductors. We argue that the anisotropic superconducting order parameter and the extremely large gap to transition temperature ratio may be associated with an unconventional pairing mechanism in the inorganic Q1D superconductor.
Thermoelectric Properties for a Suspended Microribbon of Quasi-One-Dimensional TiS3
Sakuma, Tasuku; Nishino, Shunsuke; Miyata, Masanobu; Koyano, Mikio
2018-06-01
Transition-metal trichalcogenides MX3 (M = Ti, Zr, Nb, Ta; X = S, Se) are well-known inorganic quasi-one-dimensional conductors. Among them, we have investigated the thermoelectric properties of titanium trisulfide TiS3 microribbon. The electrical resistivity ρ, thermal conductivity κ, and thermoelectric power S were measured using 3 ω method. The weight mean values were found to be ρ = 5 mω m and κ = 10 W K-1 m-1 along the one-dimensional direction ( b-axis) of the TiS3 microribbon. Combined with the thermoelectric power S = -530 μV K-1, the figure of merit was calculated as ZT = 0.0023. This efficiency is the same as that of randomly oriented bulk TiS3. We also estimated the anisotropy of σ and κ using the present results and those for randomly oriented bulk material. The obtained weak anisotropy for TiS3 is attributable to strong coupling between triangular columns consisting of TiS3 units. These experimental results are consistent with theoretical results obtained using density functional theory (DFT) calculations.
Quasi-one-dimensional density of states in a single quantum ring.
Kim, Heedae; Lee, Woojin; Park, Seongho; Kyhm, Kwangseuk; Je, Koochul; Taylor, Robert A; Nogues, Gilles; Dang, Le Si; Song, Jin Dong
2017-01-05
Generally confinement size is considered to determine the dimensionality of nanostructures. While the exciton Bohr radius is used as a criterion to define either weak or strong confinement in optical experiments, the binding energy of confined excitons is difficult to measure experimentally. One alternative is to use the temperature dependence of the radiative recombination time, which has been employed previously in quantum wells and quantum wires. A one-dimensional loop structure is often assumed to model quantum rings, but this approximation ceases to be valid when the rim width becomes comparable to the ring radius. We have evaluated the density of states in a single quantum ring by measuring the temperature dependence of the radiative recombination of excitons, where the photoluminescence decay time as a function of temperature was calibrated by using the low temperature integrated intensity and linewidth. We conclude that the quasi-continuous finely-spaced levels arising from the rotation energy give rise to a quasi-one-dimensional density of states, as long as the confined exciton is allowed to rotate around the opening of the anisotropic ring structure, which has a finite rim width.
McDermott, Danielle; Olson Reichhardt, Cynthia J; Reichhardt, Charles
2016-10-19
Using computer simulations, we study a two-dimensional system of sterically interacting self-mobile run-and-tumble disk-shaped particles with an underlying periodic quasi-one-dimensional asymmetric substrate, and show that a rich variety of collective active ratchet behaviors arise as a function of particle density, activity, substrate period, and the maximum force exerted by the substrate. The net dc drift, or ratchet transport flux, is nonmonotonic since it increases with increased activity but is diminished by the onset of self-clustering of the active particles. Increasing the particle density decreases the ratchet transport flux for shallow substrates but increases the ratchet transport flux for deep substrates due to collective hopping events. At the highest particle densities, the ratchet motion is destroyed by a self-jamming effect. We show that it is possible to realize reversals of the direction of the net dc drift in the deep substrate limit when multiple rows of active particles can be confined in each substrate minimum, permitting emergent particle-like excitations to appear that experience an inverted effective substrate potential. We map out a phase diagram of the forward and reverse ratchet effects as a function of the particle density, activity, and substrate properties.
Colloid-colloid hydrodynamic interaction around a bend in a quasi-one-dimensional channel.
Liepold, Christopher; Zarcone, Ryan; Heumann, Tibor; Rice, Stuart A; Lin, Binhua
2017-07-01
We report a study of how a bend in a quasi-one-dimensional (q1D) channel containing a colloid suspension at equilibrium that exhibits single-file particle motion affects the hydrodynamic coupling between colloid particles. We observe both structural and dynamical responses as the bend angle becomes more acute. The structural response is an increasing depletion of particles in the vicinity of the bend and an increase in the nearest-neighbor separation in the pair correlation function for particles on opposite sides of the bend. The dynamical response monitored by the change in the self-diffusion [D_{11}(x)] and coupling [D_{12}(x)] terms of the pair diffusion tensor reveals that the pair separation dependence of D_{12} mimics that of the pair correlation function just as in a straight q1D channel. We show that the observed behavior is a consequence of the boundary conditions imposed on the q1D channel: both the single-file motion and the hydrodynamic flow must follow the channel around the bend.
Two dimensionality in quasi-one-dimensional cobalt oxides confirmed by muon-spin spectroscopy
International Nuclear Information System (INIS)
Sugiyama, J.; Nozaki, H.; Ikedo, Y.; Mukai, K.; Andreica, D.; Amato, A.; Brewer, J.H.; Ansaldo, E.J.; Morris, G.D.; Takami, T.; Ikuta, H.
2007-01-01
The quasi-one-dimensional (Q1D) cobalt oxides, A n+2 Co n+1 O 3n+3 (A=Ca, Sr and Ba, n=1-∼), were investigated by muon-spin spectroscopy under applied pressures of up to 1.1GPa. The relationship between the onset Neel temperature T N on and the inter-chain distance (d ic ), which increases monotonically with n, is well fitted by the formula T N /T N,0 =(1-d ic /d ic,0 ) β . The T N on -d ic curve also predicts a large P dependence of T N for the compounds with n>=5, i.e., in the vicinity of d ic,0 , while the n=1-4 compounds show only a very small effect. Indeed, our high-pressure μ + SR results show that T N of BaCoO 3 (n=∼) is enhanced by P, with a slope of 2.1 K/GPa, whereas no detectable changes between ambient pressure and 1.0 GPa for both Ca 3 Co 2 O 6 (n=1) and Sr 4 Co 3 O 9 (n=2). This clearly confirms the role of the 2D-AF interaction on T N on in the Q1D cobalt oxides
A quasi-one-dimensional theory of sound propagation in lined ducts with mean flow
Dokumaci, Erkan
2018-04-01
Sound propagation in ducts with locally-reacting liners has received the attention of many authors proposing two- and three-dimensional solutions of the convected wave equation and of the Pridmore-Brown equation. One-dimensional lined duct models appear to have received less attention. The present paper proposes a quasi-one-dimensional theory for lined uniform ducts with parallel sheared mean flow. The basic assumption of the theory is that the effects of refraction and wall compliance on the fundamental mode remain within ranges in which the acoustic fluctuations are essentially uniform over a duct section. This restricts the model to subsonic low Mach numbers and Helmholtz numbers of less than about unity. The axial propagation constants and the wave transfer matrix of the duct are given by simple explicit expressions and can be applied with no-slip, full-slip or partial slip boundary conditions. The limitations of the theory are discussed and its predictions are compared with the fundamental mode solutions of the convected wave equation, the Pridmore-Brown equation and measurements where available.
Colloid-Colloid Hydrodynamic Interaction Around a Bend in a Quasi-One-Dimensional Channel
Liepold, Christopher; Zarcone, Ryan; Heumann, Tibor; Lin, Binhua; Rice, Stuart
We report a study of the correlation between a pair of particles in a colloid suspension in a bent quasi-one-dimensional (q1d) channel as a function of bend angle. As the bend angle becomes more acute, we observe an increasing depletion of particles in the vicinity of the bend and an increase in the nearest-neighbor separation in the pair correlation function for particles on opposite sides of the bend. Further, we observe that the peak value of D12, the coupling term in the pair diffusion tensor that characterizes the effect of the motion of particle 1 on particle 2, coincides with the first peak in the pair correlation function, and that the pair separation dependence of D12 mimics that of the pair correlation function. We show that the observed behavior is a consequence of the geometric constraints imposed by the single-file requirement that the particle centers lie on the centerline of the channel and the requirement that the hydrodynamic flow must follow the channel around the bend. We find that the correlation between a pair of particles in a colloidal suspension in a bent q1D channel has the same functional dependence on the pair correlation function as in a straight q1D channel when measured in a coordinate system that follows the centerline of the bent channel. NSF MRSEC (DMR-1420709), Dreyfus Foundation (SI-14-014).
Thermoelectric Properties for a Suspended Microribbon of Quasi-One-Dimensional TiS3
Sakuma, Tasuku; Nishino, Shunsuke; Miyata, Masanobu; Koyano, Mikio
2018-02-01
Transition-metal trichalcogenides MX3 (M = Ti, Zr, Nb, Ta; X = S, Se) are well-known inorganic quasi-one-dimensional conductors. Among them, we have investigated the thermoelectric properties of titanium trisulfide TiS3 microribbon. The electrical resistivity ρ, thermal conductivity κ, and thermoelectric power S were measured using 3ω method. The weight mean values were found to be ρ = 5 mω m and κ = 10 W K-1 m-1 along the one-dimensional direction (b-axis) of the TiS3 microribbon. Combined with the thermoelectric power S = -530 μV K-1, the figure of merit was calculated as ZT = 0.0023. This efficiency is the same as that of randomly oriented bulk TiS3. We also estimated the anisotropy of σ and κ using the present results and those for randomly oriented bulk material. The obtained weak anisotropy for TiS3 is attributable to strong coupling between triangular columns consisting of TiS3 units. These experimental results are consistent with theoretical results obtained using density functional theory (DFT) calculations.
Yoshino, Harukazu; Saito, Kazuya; Nishikawa, Hiroyuki; Kikuchi, Koichi; Kobayashi, Keiji; Ikemoto, Isao
1997-08-01
Comparative study is presented for the in-plane angular effect of magnetoresistance of quasi-one-dimensional organic conductors, (DMET)2AuBr2 and (TMTSF)2ClO4. The magnetoresistance for the magnetic and electrical fields parallel and perpendicular to the most conducting plane, respectively, was measured at 4.2 K and up to 7.0 T. (DMET)2AuBr2 shows an anomalous hump in the field-orientation dependence of the magnetoresistance for the magnetic field nearly parallel to the most conducting axis and this is very similar to what previously reported for (DMET)2I3. Weak anomaly was detected for the magnetoresistance of (TMTSF)2ClO4 in the Relaxed state, while no anomaly was observed in the SDW phase in the Quenched state. By comparing the numerical angular derivatives of the magnetoresistance, it is shown that the anomaly in the in-plane angular effect continuously develops from zero magnetic field and is closely related to the quasi-one-dimensional Fermi surface. A simple method is proposed to estimate the anisotropy of the transfer integral from the width of the hump anomaly.
DEFF Research Database (Denmark)
Claessen, R.; Sing, M.; Schwingenschlogl, U.
2002-01-01
The electronic structure of the quasi-one-dimensional organic conductor TTF-TCNQ is studied by angle-resolved photoelectron spectroscopy (ARPES). The experimental spectra reveal significant discrepancies to band theory. We demonstrate that the measured dispersions can be consistently mapped onto...
Rousse, G.; Rodríguez-Carvajal, J.; Giacobbe, C.; Sun, M.; Vaccarelli, O.; Radtke, G.
2017-04-01
A thorough structural exploration has been made on the quasi-one-dimensional S =1 /2 compound L i2C u2O (SO4) 2 by neutron and synchrotron x-ray diffraction. It reveals the occurrence of a structural transition at 125 K, characterized by a lowering of symmetry from P 42/m to P 1 ¯ , which is possibly driven by an exchange striction mechanism. This transition involves a dimerization of some Cu in the edge-sharing tetrahedral Cu chains. A symmetry mode analysis indicates that one representation, Γ3+Γ4+ , dominates the structural transition. Interestingly, no intermediate structure with P 112 /m symmetry is observed experimentally. Lastly, temperature dependent magnetic susceptibility measurements and neutron diffraction reveal that the magnetic ground state of this compound is a spin-singlet with a spin gap, characterized by the absence of long-range magnetic order down to 1.7 K.
International Nuclear Information System (INIS)
Cockburn, S. P.; Gallucci, D.; Proukakis, N. P.
2011-01-01
The stochastic Gross-Pitaevskii equation is shown to be an excellent model for quasi-one-dimensional Bose gas experiments, accurately reproducing the in situ density profiles recently obtained in the experiments of Trebbia et al.[Phys. Rev. Lett. 97, 250403 (2006)] and van Amerongen et al.[Phys. Rev. Lett. 100, 090402 (2008)] and the density fluctuation data reported by Armijo et al.[Phys. Rev. Lett. 105, 230402 (2010)]. To facilitate such agreement, we propose and implement a quasi-one-dimensional extension to the one-dimensional stochastic Gross-Pitaevskii equation for the low-energy, axial modes, while atoms in excited transverse modes are treated as independent ideal Bose gases.
Directory of Open Access Journals (Sweden)
Yuriy Kruglyak
2015-06-01
Full Text Available This review is devoted to the basic problem in quantum theory of quasi-one-dimensional electron systems like polyenes (Part 1 and cumulenes (Part 2 – physical origin of the forbidden zone in these and analogous 1D electron systems due to two possible effects – Peierls instability (bond alternation and Mott instability (electron correlation. Both possible contradiction and coexistence of the Mott and Peierls instabilities are summerized on the basis of the Kiev quantum chemistry team research projects.
Magnetic behaviour of interacting antiferromagnetic nanoparticles
International Nuclear Information System (INIS)
Markovich, V; Jung, G; Gorodetsky, G; Puzniak, R; Wisniewski, A; Skourski, Y; Mogilyanski, D
2012-01-01
Magnetic properties of interacting La 0.2 Ca 0.8 MnO 3 nanoparticles have been investigated. The field-induced transition from antiferromagnetic (AFM) to ferromagnetic (FM) state in the La 0.2 Ca 0.8 MnO 3 bulk has been observed at exceptionally high magnetic fields. For large particles, the field-induced transition widens while magnetization progressively decreases. In small particles the transition is almost fully suppressed. The thermoremanence and isothermoremanence curves constitute fingerprints of irreversible magnetization originating from nanoparticle shells. We have ascribed the magnetic behaviour of nanoparticles to a core-shell scenario with two main magnetic contributions; one attributed to the formation of a collective state formed by FM clusters in frustrated coordination at the surfaces of interacting AFM nanoparticles and the other associated with inner core behaviour as a two-dimensional diluted antiferromagnet. (paper)
Thermoinduced magnetization in nanoparticles of antiferromagnetic materials
DEFF Research Database (Denmark)
Mørup, Steen; Frandsen, Cathrine
2004-01-01
We show that there is a thermoinduced contribution to the magnetic moment of nanoparticles of antiferromagnetic materials. It arises from thermal excitations of the uniform spin-precession mode, and it has the unusual property that its magnitude increases with increasing temperature. This has...
A neutron scattering study of the quasi-one-dimensional conductor (TaSe{sub 4}){sub 2}I
Energy Technology Data Exchange (ETDEWEB)
Lorenzo, J.E.; Currat, R. [Institut Laue-Langevin, BP 156, 38042 Grenoble Cedex 9 (France); Monceau, P. [Centre de Recherches sur les Tres Basses Temperatures, associe a l' Universite Joseph Fourier, CNRS, BP 166, 38042 Grenoble Cedex 9 (France); Hennion, B. [Laboratoire Leon Brillouin, Centre d' Etudes de Saclay, 91191 Gif-sur-Yvette Cedex (France); Berger, H.; Levy, F. [Institut de Physique Appliquee, Ecole Polytechnique Federale de Lausanne, CH-1015 Lausanne (Switzerland)
1998-06-15
The Peierls phase transition in the quasi-one-dimensional conductor (TaSe{sub 4}){sub 2}I is investigated by means of elastic and inelastic neutron scattering. The effective critical exponent {beta}, extracted from the temperature dependence of the integrated intensity from the CDW satellite reflections, is anomalously low, suggesting that the phase transition may be of first order. The intensity distribution among symmetry-related satellite reflections indicates a domain structure with slowly fluctuating domain populations. Correlation lengths associated with the diverging 'central peak' are determined and are found to be nearly isotropic, at variance with results obtained on other quasi-one-dimensional compounds, such as platinum chains (KCP) or blue bronze, K{sub 0.3}MoO{sub 3}. Doping with 1.2% Nb has a severe effect on the modulated state. The low-temperature satellites are replaced by a diffuse scattering distribution elongated along c*. The absence of a phonon soft mode and the presence of a diverging central peak at the phase transition is interpreted within the framework of strong electron-phonon coupling. Finally, we propose a Ginzburg-Landau phenomenological model, where the interplay between the electronically coupled optical-like order parameter (Ta-atom tetramerization along the chain axis) and the elastic deformations lies at the origin of the phase transition in (TaSe{sub 4}){sub 2}I. (author)
International Nuclear Information System (INIS)
Levin, B.N.
1984-01-01
The propagation of an inhomogeneous stream of fast electrons through the corona - the type III radio burst source - is considered. It is shown, that the angular spectrum width of plasma waves excited by the stream is defined both by Landau damping by particles of the diffuse component and by damping (in the region of large phase velocities) by particles of the stream itself having large pitch angles. The regime of quasi-one-dimensional diffusion in the velocity space is realized only in the presence of a sufficiently dense diffuse component of super-thermal particles and only for a sufficiently large inhomogeneity scale of the stream. A large scale of the stream space profile is formed, evidently, close to the region of injection of super-thermal particles. It is the result of 'stripping' of part of the electrons from the stream front to its slower part due to essential non-one-dimensionality of the particle diffusion in velocity space. Results obtained may explain, in particular, the evolution of a stream particle angular spectrum in the generation region of type III radio bursts observed by spacecrafts (Lin et al., 1981). For the relatively low energetic part of the stream, the oblique plasma wave stabilization by a diffuse component results in a quasi-one-dimensional regime of diffusion. The latter conserves the beam-like structure of this part of the stream. (orig.)
Neutron diffraction study of quasi-one-dimensional spin-chain ...
Indian Academy of Sciences (India)
The high temperature magnetic susceptibility obeys the Curie–Weiss law; the value of the paramagnetic Curie temperature () decreases as the concentration of iron increases and it becomes negative for = 0.4. No extra Bragg peak as well as no observable enhancement in the intensity of the fundamental (nuclear) ...
Multichain Mean-Field Theory of Quasi-One-Dimensional Quantum Spin Systems
International Nuclear Information System (INIS)
Sandvik, A.W.
1999-01-01
A multichain mean-field theory is developed and applied to a two-dimensional system of weakly coupled S=1/2 Heisenberg chains. The environment of a chain C 0 is modeled by a number of neighboring chains C δ , δ=±1, hor-ellipsis,± , with the edge chains C ±n coupled to a staggered field. Using a quantum Monte Carlo method, the effective (2n+1) -chain Hamiltonian is solved self-consistently for n up to 4 . The results are compared with simulation results for the original Hamiltonian on large rectangular lattices. Both methods show that the staggered magnetization M for small interchain couplings α behaves as M∼√(α) enhanced by a multiplicative logarithmic correction. copyright 1999 The American Physical Society
Resistively detected NMR line shapes in a quasi-one-dimensional electron system
Fauzi, M. H.; Singha, A.; Sahdan, M. F.; Takahashi, M.; Sato, K.; Nagase, K.; Muralidharan, B.; Hirayama, Y.
2017-06-01
We observe variation in the resistively detected nuclear magnetic resonance (RDNMR) line shapes in quantum Hall breakdown. The breakdown occurs locally in a gate-defined quantum point contact (QPC) region. Of particular interest is the observation of a dispersive line shape occurring when the bulk two-dimensional electron gas (2DEG) set to νb=2 and the QPC filling factor to the vicinity of νQPC=1 , strikingly resemble the dispersive line shape observed on a 2D quantum Hall state. This previously unobserved line shape in a QPC points to a simultaneous occurrence of two hyperfine-mediated spin flip-flop processes within the QPC. Those events give rise to two different sets of nuclei polarized in the opposite direction and positioned at a separate region with different degrees of electronic spin polarization.
X-ray photoelectron spectra and electronic structure of quasi-one-dimensional SbSeI crystals
Directory of Open Access Journals (Sweden)
J.Grigas
2007-01-01
Full Text Available The paper presents the X-ray photoelectron spectra (XPS of the valence band (VB and of the principal core levels from the (110 and (001 crystal surfaces for the quasi-one-dimensional high permittivity SbSeI single crystal isostructural to ferroelectric SbSI. The XPS were measured with monochromatized Al Ka radiation in the energy range of 0-1400 eV at room temperature. The VB is located from 1.6 to 20 eV below the Fermi level. Experimental energies of the VB and core levels are compared with the results of theoretical ab initio calculations of the molecular model of the SbSeI crystal. The electronic structure of the VB is revealed. Shifts in the core-level binding energies of surface atoms relative to bulk ones, which show a dependency on surface crystallography, have been observed. The chemical shifts of the core levels (CL in the SbSeI crystal for the Sb, I and Se states are obtained.
Gildfind, D. E.; Jacobs, P. A.; Morgan, R. G.; Chan, W. Y. K.; Gollan, R. J.
2017-11-01
Large-scale free-piston driven expansion tubes have uniquely high total pressure capabilities which make them an important resource for development of access-to-space scramjet engine technology. However, many aspects of their operation are complex, and their test flows are fundamentally unsteady and difficult to measure. While computational fluid dynamics methods provide an important tool for quantifying these flows, these calculations become very expensive with increasing facility size and therefore have to be carefully constructed to ensure sufficient accuracy is achieved within feasible computational times. This study examines modelling strategies for a Mach 10 scramjet test condition developed for The University of Queensland's X3 facility. The present paper outlines the challenges associated with test flow reconstruction, describes the experimental set-up for the X3 experiments, and then details the development of an experimentally tuned quasi-one-dimensional CFD model of the full facility. The 1-D model, which accurately captures longitudinal wave processes, is used to calculate the transient flow history in the shock tube. This becomes the inflow to a higher-fidelity 2-D axisymmetric simulation of the downstream facility, detailed in the Part 2 companion paper, leading to a validated, fully defined nozzle exit test flow.
Anisotropic transport in the quasi-one-dimensional semiconductor Li{sub 0.33}MoO{sub 3}
Energy Technology Data Exchange (ETDEWEB)
Moshfeghyeganeh, S.; Cote, A. N.; Cohn, J. L., E-mail: cohn@physics.miami.edu [Department of Physics, University of Miami, Coral Gables, Florida 33124 (United States); Neumeier, J. J. [Department of Physics, Montana State University, Bozeman, Montana 59717 (United States)
2016-03-07
Transport measurements (electrical resistivity, Seebeck coefficient, and thermal conductivity) in the temperature range 80–500 K are presented for single crystals of the quasi-one-dimensional (Q1D) semiconductor Li{sub 0.33}MoO{sub 3}. Opposite signs are observed for the Seebeck coefficient along the trinclinic a and c axes, with S{sub c} − S{sub a} ≃ 250 μV/K near room temperature and ≃100 μV/K at 380 K. The thermal conductivity at room temperature in the a-c planes was ∼2 W/m K and ∼10 times smaller along b*. A weak structural anomaly at T{sub s} ≈ 355 K, identified in the temperature-dependent lattice constants, coincides with anomalies in the electrical properties. Analysis of the electronic transport at T > T{sub s} favors an intrinsic semiconductor picture for transport along the most conducting Q1D axis and small-polaronic transport along the other directions, providing insight into the origin of the Seebeck anisotropy.
Gildfind, D. E.; Jacobs, P. A.; Morgan, R. G.; Chan, W. Y. K.; Gollan, R. J.
2018-07-01
Large-scale free-piston driven expansion tubes have uniquely high total pressure capabilities which make them an important resource for development of access-to-space scramjet engine technology. However, many aspects of their operation are complex, and their test flows are fundamentally unsteady and difficult to measure. While computational fluid dynamics methods provide an important tool for quantifying these flows, these calculations become very expensive with increasing facility size and therefore have to be carefully constructed to ensure sufficient accuracy is achieved within feasible computational times. This study examines modelling strategies for a Mach 10 scramjet test condition developed for The University of Queensland's X3 facility. The present paper outlines the challenges associated with test flow reconstruction, describes the experimental set-up for the X3 experiments, and then details the development of an experimentally tuned quasi-one-dimensional CFD model of the full facility. The 1-D model, which accurately captures longitudinal wave processes, is used to calculate the transient flow history in the shock tube. This becomes the inflow to a higher-fidelity 2-D axisymmetric simulation of the downstream facility, detailed in the Part 2 companion paper, leading to a validated, fully defined nozzle exit test flow.
Kiefer, Thomas; Villanueva, Guillermo; Brugger, Jürgen
2009-08-01
In this study we investigate electrical conduction in finite rectangular random resistor networks in quasione and two dimensions far away from the percolation threshold p(c) by the use of a bond percolation model. Various topologies such as parallel linear chains in one dimension, as well as square and triangular lattices in two dimensions, are compared as a function of the geometrical aspect ratio. In particular we propose a linear approximation for conduction in two-dimensional systems far from p(c), which is useful for engineering purposes. We find that the same scaling function, which can be used for finite-size scaling of percolation thresholds, also applies to describe conduction away from p(c). This is in contrast to the quasi-one-dimensional case, which is highly nonlinear. The qualitative analysis of the range within which the linear approximation is legitimate is given. A brief link to real applications is made by taking into account a statistical distribution of the resistors in the network. Our results are of potential interest in fields such as nanostructured or composite materials and sensing applications.
International Nuclear Information System (INIS)
Rozhkov, A.V.
2007-01-01
A mechanism for superconductivity in a quasi-one-dimensional system with repulsive Ising-anisotropic interaction is studied. The Ising anisotropy opens the gap Δ s in the spin sector of the model. This gap allows the triplet superconductivity and the spin-density wave as the only broken symmetry phases. These phases are separated by the first order transition. The transport properties of the system are investigated in different parts of the phase diagram. The calculation of DC conductivity σ(T) in the high-temperature phase shows that the function σ(T) cannot be used as an indicator of a superconducting ground state: even if σ(T) is a decreasing function at high temperature, yet, the ground state may be insulating spin-density wave; the opposite is also true. The calculation of the spin dynamical structure factor S zz (q, ω) demonstrates that it is affected by the superconducting phase transition in a qualitative fashion: below T c the structure factor develops a gap with a coherent excitation inside this gap
International Nuclear Information System (INIS)
Gasparian, Vladimir; Cahay, Marc; Jodar, Esther
2011-01-01
A two-dimensional δ-potential Kronig-Penney model for quasi-one-dimensional (Q1D) disordered systems is used to study analytically the influence of a constant electric field on the inverse localization length (LL). Based on the Green's function formalism we have calculated LL as a function of the incoming energy E, electric field F, length L of the Q1D sample, number of modes M in the transverse direction and the amount of disorder w. We show that, for large L in Q1D systems, states are weakly localized, i.e. we deal with power-law localization. With increasing electric field in Q1D mesoscopic systems a transition from exponential to a power-law behavior takes place, as in 1D systems. We note that the graphs showing the inverse LL change significantly with increasing F (for fixed M) rather than with increasing M (for fixed F). We also show that the graphs representing the ratio of the corresponding localization length without and with electric field collapse for all modes M into a universal curve in the Q1D strip model.
International Nuclear Information System (INIS)
Nobile, A.; Tosatti, E.
1979-05-01
The coexistence of tight-binding and exchange-correlation effects inside each chain of a model quasi-one-dimensional metal, on both plasmon and charge density wave properties have been studied. The results, while in qualitative agreement with other treatments of the problem at long wavelengths, indicate a strong tendency for plasmons to turn into excitons at larger momenta, and to exhibit an ''excitonic'' charge-density wave instability at k approximately 2ksub(F). The nature of the plasmon branches and of the excitonic charge distortion is examined. Relevance to existing quasi-one-dimensional materials is also discussed. (author)
Dessup, Tommy; Coste, Christophe; Saint Jean, Michel
2016-01-01
In this article, we study the effects of white Gaussian additive thermal noise on a subcritical pitchfork bifurcation. We consider a quasi-one-dimensional system of particles that are transversally confined, with short-range (non-Coulombic) interactions and periodic boundary conditions in the longitudinal direction. In such systems, there is a structural transition from a linear order to a staggered row, called the zigzag transition. There is a finite range of transverse confinement stiffnesses for which the stable configuration at zero temperature is a localized zigzag pattern surrounded by aligned particles, which evidences the subcriticality of the bifurcation. We show that these configurations remain stable for a wide temperature range. At zero temperature, the transition between a straight line and such localized zigzag patterns is hysteretic. We have studied the influence of thermal noise on the hysteresis loop. Its description is more difficult than at T =0 K since thermally activated jumps between the two configurations always occur and the system cannot stay forever in a unique metastable state. Two different regimes have to be considered according to the temperature value with respect to a critical temperature Tc(τobs) that depends on the observation time τobs. An hysteresis loop is still observed at low temperature, with a width that decreases as the temperature increases toward Tc(τobs) . In contrast, for T >Tc(τobs) the memory of the initial condition is lost by stochastic jumps between the configurations. The study of the mean residence times in each configuration gives a unique opportunity to precisely determine the barrier height that separates the two configurations, without knowing the complete energy landscape of this many-body system. We also show how to reconstruct the hysteresis loop that would exist at T =0 K from high-temperature simulations.
Isostructural magnetic phase transition and magnetocaloric effect in Ising antiferromagnet
International Nuclear Information System (INIS)
Lavanov, G.Yu; Kalita, V.M.; Loktev, V.M.
2014-01-01
It is shown that the external magnetic field induced isostructural I st order magnetic phase transition between antiferromagnetic phases with different antiferromagnetic vector values is associated with entropy. It is found, that depending on temperature the entropy jump and the related heat release change their sign at this transition point. In the low-temperature region of metamagnetic I st order phase tensition the entropy jump is positive, and in the triple point region this jump for isostructural magnetic transition is negative
Physical Properties of (NH4)2Pt(CN)4[Clo.42].3H2O: A new Quasi-One-Dimensional Conductor
DEFF Research Database (Denmark)
Carneiro, Kim; Petersen, A. S.; Underhill, A. E.
1979-01-01
The quasi-one-dimensional conductor (NH4)2[Pt(CN)4]Cl0.42·3H2O, ACP(Cl), has been studied experimentally by means of electrical conduction measurements, x-ray diffuse scattering, and neutron inelastic scattering. This allows the determination of all the physical parameters of interest for the the......The quasi-one-dimensional conductor (NH4)2[Pt(CN)4]Cl0.42·3H2O, ACP(Cl), has been studied experimentally by means of electrical conduction measurements, x-ray diffuse scattering, and neutron inelastic scattering. This allows the determination of all the physical parameters of interest...
Matsumoto, Karin; Ogura, Daisuke; Kuroki, Kazuhiko
2018-01-01
We study superconductivity in the Hubbard model on various quasi-one-dimensional lattices with coexisting wide and narrow bands originating from multiple sites within a unit cell, where each site corresponds to a single orbital. The systems studied are the two-leg and three-leg ladders, the diamond chain, and the crisscross ladder. These one-dimensional lattices are weakly coupled to form two-dimensional (quasi-one-dimensional) ones, and the fluctuation exchange approximation is adopted to study spin-fluctuation-mediated superconductivity. When one of the bands is perfectly flat and the Fermi level intersecting the wide band is placed in the vicinity of, but not within, the flat band, superconductivity arising from the interband scattering processes is found to be strongly enhanced owing to the combination of the light electron mass of the wide band and the strong pairing interaction due to the large density of states of the flat band. Even when the narrow band has finite bandwidth, the pairing mechanism still works since the edge of the narrow band, due to its large density of states, plays the role of the flat band. The results indicate the wide applicability of the high-Tc pairing mechanism due to coexisting wide and "incipient" narrow bands in quasi-one-dimensional systems.
Magnetic Transport in Spin Antiferromagnets for Spintronics Applications
Directory of Open Access Journals (Sweden)
Mohamed Azzouz
2017-10-01
Full Text Available Had magnetic monopoles been ubiquitous as electrons are, we would probably have had a different form of matter, and power plants based on currents of these magnetic charges would have been a familiar scene of modern technology. Magnetic dipoles do exist, however, and in principle one could wonder if we can use them to generate magnetic currents. In the present work, we address the issue of generating magnetic currents and magnetic thermal currents in electrically-insulating low-dimensional Heisenberg antiferromagnets by invoking the (broken electricity-magnetism duality symmetry. The ground state of these materials is a spin-liquid state that can be described well via the Jordan–Wigner fermions, which permit an easy definition of the magnetic particle and thermal currents. The magnetic and magnetic thermal conductivities are calculated in the present work using the bond–mean field theory. The spin-liquid states in these antiferromagnets are either gapless or gapped liquids of spinless fermions whose flow defines a current just as the one defined for electrons in a Fermi liquid. The driving force for the magnetic current is a magnetic field with a gradient along the magnetic conductor. We predict the generation of a magneto-motive force and realization of magnetic circuits using low-dimensional Heisenberg antiferromagnets. The present work is also about claiming that what the experiments in spintronics attempt to do is trying to treat the magnetic degrees of freedoms on the same footing as the electronic ones.
On the magnetism of Heisenberg double-layer antiferromagnets
International Nuclear Information System (INIS)
Uijen, C.M.J. van.
1980-01-01
The author investigates the sublattice magnetization and the susceptibility of the double-layer Heisenberg antiferromagnet K 3 M 2 F 7 by employing the techniques of elastic and quasi-elastic critical magnetic scattering of neutrons. (G.T.H.)
Ferro- and antiferro-magnetism in (Np, Pu)BC
Czech Academy of Sciences Publication Activity Database
Klimczuk, T.; Shick, Alexander; Kozub, Agnieszka L.; Griveau, J.C.; Colineau, E.; Falmbigl, M.; Wastin, F.; Rogl, P.
2015-01-01
Roč. 3, č. 4 (2015), "041803-1"-"041803-9" ISSN 2166-532X R&D Projects: GA ČR GA15-07172S Institutional support: RVO:68378271 Keywords : ferromagetism * antiferromagnetism * magnetic anisotropy * strong electron correlations * spin-orbit coupling Subject RIV: BM - Solid Matter Physics ; Magnetism Impact factor: 4.323, year: 2015
High magnetic field magnetization of a new triangular lattice antiferromagnet
Energy Technology Data Exchange (ETDEWEB)
Zhou, H. D. [Univ. of Tennessee, Knoxville, TN (United States); Los Alamos National Lab. (LANL), Los Alamos, NM (United States). National High Magnetic Field Lab. (MagLab); Stritzinger, Laurel Elaine Winter [Los Alamos National Lab. (LANL), Los Alamos, NM (United States); Harrison, Neil [Los Alamos National Lab. (LANL), Los Alamos, NM (United States)
2017-03-23
In CsV(MoO_{4})_{2}, the magnetic V^{3+} ions with octahedral oxygen-coordination form a geometrically frustrated triangular lattice. So fare, there is no magnetic properties reported on it. Recently, we successfully grew single crystals of CsV(MoO_{4})_{2} by using flux method. The susceptibility shows a sharp drop around 24 K, representing a long range magnetic ordering. To understand the physical properties of this new triangular lattice antiferromagnet (TLAF), we pursued high field magnetization measurements to answer two questions: (i) what is the saturation field, which will be very useful to calculate the exchange interaction of the system? (ii) Will it exhibit spin state transition, such as the up up down phase with 1/3-saturation moment as other TLAFs? Recently, we performed VSM measurements in Cell 8, Tallahassee, NHMFL, the results show that the magnetization reaches 0.38 MuB at 34 T, which is just 19% of the full moment of 2 MuB for V^{3+} (3d^{2}) ions. Apparently we need higher field to reach 1/3 value or full moment.
Energy Technology Data Exchange (ETDEWEB)
Wong, C.H., E-mail: ch.kh.vong@urfu.ru [Institute of Physics and Technology, Ural Federal University, Clear Water Bay, Kowloon (Russian Federation); Wu, R.P.H., E-mail: pak-hong-raymond.wu@connect.polyu.hk [Department of Applied Physics, The Hong Kong Polytechnic University (Hong Kong); Lortz, R., E-mail: lortz@ust.hk [Department of Physics, Hong Kong University of Science and Technology (Hong Kong)
2017-03-15
The dimensional crossover from a 1D fluctuating state at high temperatures to a 3D phase coherent state in the low temperature regime in two coaxial weakly-coupled cylindrical surfaces formed by two-dimensional arrays of parallel nanowires is studied via an 8-state 3D-XY model. This system serves as a model for quasi-one-dimensional superconductors in the form of bundles of weakly-coupled superconducting nanowires. A periodic variation of the dimensional crossover temperature T{sub DC} is observed when the inner superconducting cylindrical surface is rotated in the angular plane. T{sub DC} reaches a maximum when the relative angle between the cylinders is 2.81°, which corresponds to the maximum separation of nanowires between the two cylindrical surfaces. We demonstrate that the relative strength of phase fluctuations in this system is controllable by the rotational angle between the two surfaces with a strong suppression of the fluctuation strength at 2.81°. The phase fluctuations are suppressed gradually upon cooling, before they abruptly vanish below T{sub DC}. Our model thus allows us to study how phase fluctuations can be suppressed in quasi-one-dimensional superconductors in order to achieve a global phase coherent state throughout the nanowire array with zero electric resistance.
Highly tunable perpendicularly magnetized synthetic antiferromagnets for biotechnology applications
Vemulkar, T; Mansell, Rhodri; Petit, Dorothee Celine; Cowburn, Russell Paul; Lesniak, MS
2015-01-01
Magnetic micro and nanoparticles are increasingly used in biotechnological applications due to the ability to control their behavior through an externally applied field. We demonstrate the fabrication of particles made from ultrathin perpendicularly magnetized CoFeB/Pt layers with antiferromagnetic interlayer coupling. The particles are characterized by zero moment at remanence, low susceptibility at low fields, and a large saturated moment created by the stacking of the basic coupled bilayer...
Directory of Open Access Journals (Sweden)
D. H. Berman
2014-03-01
Full Text Available Resonant behavior involving spin-orbit entangled states occurs for spin transport along a narrow channel defined in a two-dimensional electron gas, including an apparent rapid relaxation of the spin polarization for special values of the channel width and applied magnetic field (so-called ballistic spin resonance. A fully quantum-mechanical theory for transport using multiple subbands of the one-dimensional system provides the dependence of the spin density on the applied magnetic field and channel width and position along the channel. We show how the spatially nonoscillating part of the spin density vanishes when the Zeeman energy matches the subband energy splittings. The resonance phenomenon persists in the presence of disorder.
Dilute antiferromagnetism in magnetically doped phosphorene
Directory of Open Access Journals (Sweden)
Andrew Allerdt
2017-11-01
Full Text Available We study the competition between Kondo physics and indirect exchange on monolayer black phos-phorous using a realistic description of the band structure in combination with the density matrixrenormalization group (DMRG method. The Hamiltonian is reduced to a one-dimensional problemvia an exact canonical transformation that makes it amenable to DMRG calculations, yielding exactresults that fully incorporate the many-body physics. We find that a perturbative description of theproblem is not appropriate and cannot account for the slow decay of the correlations and the completelack of ferromagnetism. In addition, at some particular distances, the impurities decouple formingtheir own independent Kondo states. This can be predicted from the nodes of the Lindhard function.Our results indicate a possible route toward realizing dilute anti-ferromagnetism in phosphorene. Received: 19 September 2017, Accepted: 12 October 2017; Edited by: K. Hallberg; DOI: http://dx.doi.org/10.4279/PIP.090008 Cite as: A Allerdt, A E Feiguin, Papers in Physics 9, 090008 (2017
Magnetization reversal in weak ferrimagnets and canted antiferromagnets
International Nuclear Information System (INIS)
Kageyama, H.; Khomskii, D.I.; Levitin, R.Z.; Markina, M.M.; Okuyama, T.; Uchimoto, T.; Vasil'ev, A.N.
2003-01-01
In some ferrimagnets the total magnetization vanishes at a certain compensation temperature T*. In weak magnetic fields, the magnetization can change sign at T* (the magnetization reversal). Much rarer is observation of ferrimagnetic-like response in canted antiferromagnets, where the weak ferromagnetic moment is due to the tilting of the sublattice magnetizations. The latter phenomenon was observed in nickel (II) formate dihydrate Ni(HCOO) 2 ·2H 2 O. The observed weak magnetic moment increases initially below T N =15.5 K, equals zero at T*=8.5 K and increases again at lowering temperature. The sign of the low-field magnetization at any given temperature is determined by the sample's magnetic prehistory and the signs are opposite to each other at T N
He, Jiaming; Zhang, Yiran; Wen, Libin; Yang, Yusen; Liu, Jinyu; Wu, Yueshen; Lian, Hailong; Xing, Hui; Wang, Shun; Mao, Zhiqiang; Liu, Ying
2017-07-01
Ta2NiSe7 is a quasi-one-dimensional (quasi-1D) transition-metal chalcogenide with Ta and Ni chain structures. An incommensurate charge-density wave (CDW) in this quasi-1D structure was well studied previously using tunnelling spectrum, X-ray, and electron diffraction, whereas its transport property and the relation to the underlying electronic states remain to be explored. Here, we report our results of the magnetoresistance (MR) on Ta2NiSe7. A breakdown of Kohler's rule is found upon entering the CDW state. Concomitantly, a clear change in curvature in the field dependence of MR is observed. We show that the curvature change is well described by the two-band orbital MR, with the hole density being strongly suppressed in the CDW state, indicating that the p orbitals from Se atoms dominate the change in transport through CDW transition.
Reichhardt, Charles; Reichhardt, Cynthia J. Olson
We numerically examine skyrmions interacting with a periodic quasi-one-dimensional substrate. When we drive the skyrmions perpendicular to the substrate periodicity direction, a rich variety of nonlinear Magnus-induced effects arise, in contrast to an overdamped system that shows only a linear velocity-force curve for this geometry. The skyrmion velocity-force curve is strongly nonlinear and we observe a Magnus-induced speed-up effect when the pinning causes the Magnus velocity response to align with the dissipative response. At higher applied drives these components decouple, resulting in strong negative differential conductivity. For skyrmions under combined ac and dc driving, we find a new class of phase locking phenomena in which the velocity-force curves contain a series of what we call Shapiro spikes, distinct from the Shapiro steps observed in overdamped systems. There are also regimes in which the skyrmion moves in the direction opposite to the applied dc drive to give negative mobility.
Energy Technology Data Exchange (ETDEWEB)
Loeffler, J.; Wagner, W.; Svygenhoven, H. van [Paul Scherrer Inst. (PSI), Villigen (Switzerland); Meier, J.; Doudin, B.; Ansermet, J.P. [Ecole Polytechnique Federale, Lausanne (Switzerland)
1997-09-01
The magnetic properties of nanostructured materials on the basis of Fe and Ni have been investigated with a SQUID magnetometer, complementary to the small-angle neutron scattering study reported in the same volume. Measurements of the coercive field in a temperature range from 5 to 300 K confirm the validity of the random anisotropy model for our nanostructured systems. Furthermore, we obtain information about the presence and distribution of the antiferromagnetic oxides, joining the ferromagnetic grains. (author) 2 figs., 3 refs.
International Nuclear Information System (INIS)
Loeffler, J.; Wagner, W.; Svygenhoven, H. van; Meier, J.; Doudin, B.; Ansermet, J.P.
1997-01-01
The magnetic properties of nanostructured materials on the basis of Fe and Ni have been investigated with a SQUID magnetometer, complementary to the small-angle neutron scattering study reported in the same volume. Measurements of the coercive field in a temperature range from 5 to 300 K confirm the validity of the random anisotropy model for our nanostructured systems. Furthermore, we obtain information about the presence and distribution of the antiferromagnetic oxides, joining the ferromagnetic grains. (author) 2 figs., 3 refs
Singlet Ground State Magnetism: III Magnetic Excitons in Antiferromagnetic TbP
DEFF Research Database (Denmark)
Knorr, K.; Loidl, A.; Kjems, Jørgen
1981-01-01
The dispersion of the lowest magnetic excitations of the singlet ground state system TbP has been studied in the antiferromagnetic phase by inelastic neutron scattering. The magnetic exchange interaction and the magnetic and the rhombohedral molecular fields have been determined.......The dispersion of the lowest magnetic excitations of the singlet ground state system TbP has been studied in the antiferromagnetic phase by inelastic neutron scattering. The magnetic exchange interaction and the magnetic and the rhombohedral molecular fields have been determined....
Ground State of Quasi-One Dimensional Competing Spin Chain Cs2Cu2Mo3O12 at zero and Finite Fields
Matsui, Kazuki; Goto, Takayuki; Angel, Julia; Watanabe, Isao; Sasaki, Takahiko; Hase, Masashi
The ground state of competing-spin-chain Cs2Cu2Mo3O12 with the ferromagnetic exchange interaction J1 = -93 K on nearest-neighboring spins and the antiferromagnetic one J2 = +33 K on next-nearest-neighboring spins was investigated by ZF/LF-μSR and 133Cs-NMR in the 3He temperature range. The zero-field μSR relaxation rate λ shows a significant increase below 1.85 K, suggesting the existence of magnetic order, which is consistent with the recent report on the specific heat. However, LF decoupling data at the lowest temperature 0.3 K indicate that the spins fluctuate dynamically, suggesting that the system is in a quasi-static ordered state under zero field. This idea is further supported by the fact that the broadening in NMR spectra below TN is weakened at low field below 2 T.
Low Field Magnetic and Thermal Hysteresis in Antiferromagnetic Dysprosium
Directory of Open Access Journals (Sweden)
Iuliia Liubimova
2017-06-01
Full Text Available Magnetic and thermal hysteresis (difference in magnetic properties on cooling and heating have been studied in polycrystalline Dy (dysprosium between 80 and 250 K using measurements of the reversible Villari effect and alternating current (AC susceptibility. We argue that measurement of the reversible Villari effect in the antiferromagnetic phase is a more sensitive method to detect magnetic hysteresis than the registration of conventional B(H loops. We found that the Villari point, recently reported in the antiferromagnetic phase of Dy at 166 K, controls the essential features of magnetic hysteresis and AC susceptibility on heating from the ferromagnetic state: (i thermal hysteresis in AC susceptibility and in the reversible Villari effect disappears abruptly at the temperature of the Villari point; (ii the imaginary part of AC susceptibility is strongly frequency dependent, but only up to the temperature of the Villari point; (iii the imaginary part of the susceptibility drops sharply also at the Villari point. We attribute these effects observed at the Villari point to the disappearance of the residual ferromagnetic phase. The strong influence of the Villari point on several magnetic properties allows this temperature to be ranked almost as important as the Curie and Néel temperatures in Dy and likely also for other rare earth elements and their alloys.
Metallic magnets without inversion symmetry and antiferromagnetic quantum critical points
Energy Technology Data Exchange (ETDEWEB)
Fischer, I.A.
2006-07-01
This thesis focusses on two classes of systems that exhibit non-Fermi liquid behaviour in experiments: we investigated aspects of chiral ferromagnets and of antiferromagnetic metals close to a quantum critical point. In chiral ferromagnets, the absence of inversion symmetry makes spin-orbit coupling possible, which leads to a helical modulation of the ferromagnetically ordered state. We studied the motion of electrons in the magnetically ordered state of a metal without inversion symmetry by calculating their generic band-structure. We found that spin-orbit coupling, although weak, has a profound effect on the shape of the Fermi surface: On a large portion of the Fermi surface the electron motion parallel to the helix practically stops. Signatures of this effect can be expected to show up in measurements of the anomalous Hall effect. Recent neutron scattering experiments uncovered the existence of a peculiar kind of partial order in a region of the phase diagram adjacent to the ordered state of the chiral ferromagnet MnSi. Starting from the premise that this partially ordered state is a thermodynamically distinct phase, we investigated an extended Ginzburg-Landau theory for chiral ferromagnets. In a certain parameter regime of the Ginzburg-Landau theory we identified crystalline phases that are reminiscent of the so-called blue phases in liquid crystals. Many antiferromagnetic heavy-fermion systems can be tuned into a regime where they exhibit non-Fermi liquid exponents in the temperature dependence of thermodynamic quantities such as the specific heat capacity; this behaviour could be due to a quantum critical point. If the quantum critical behaviour is field-induced, the external field does not only suppress antiferromagnetism but also induces spin precession and thereby influences the dynamics of the order parameter. We investigated the quantum critical behavior of clean antiferromagnetic metals subject to a static, spatially uniform external magnetic field. We
Cai, Kai; Liu, Jiawei; Zhang, Huan; Huang, Zhao; Lu, Zhicheng; Foda, Mohamed F; Li, Tingting; Han, Heyou
2015-05-11
An intermediate-template-directed method has been developed for the synthesis of quasi-one-dimensional Au/PtAu heterojunction nanotubes by the heterogeneous nucleation and growth of Au on Te/Pt core-shell nanostructures in aqueous solution. The synthesized porous Au/PtAu bimetallic nanotubes (PABNTs) consist of porous tubular framework and attached Au nanoparticles (AuNPs). The reaction intermediates played an important role in the preparation, which fabricated the framework and provided a localized reducing agent for the reduction of the Au and Pt precursors. The Pt7 Au PABNTs showed higher electrocatalytic activity and durability in the oxygen-reduction reaction (ORR) in 0.1 M HClO4 than porous Pt nanotubes (PtNTs) and commercially available Pt/C. The mass activity of PABNTs was 218 % that of commercial Pt/C after an accelerated durability test. This study demonstrates the potential of PABNTs as highly efficient electrocatalysts. In addition, this method provides a facile strategy for the synthesis of desirable hetero-nanostructures with controlled size and shape by utilizing an intermediate template. © 2015 WILEY-VCH Verlag GmbH & Co. KGaA, Weinheim.
On the control parameters of the quasi-one dimensional superconductivity in Sc{sub 3}CoC{sub 4}
Energy Technology Data Exchange (ETDEWEB)
Eickerling, Georg; Hauf, Christoph; Scheidt, Ernst-Wilhelm; Reichardt, Lena; Schneider, Christian; Scherer, Wolfgang [Institut fuer Physik, Universitaet Augsburg, Universitaetstrasse 1, 86179 Augsburg (Germany); Munoz, Alfonso [Departamento de Fisica Fundamental II, Instituto de Materiales y Nanotecnologia, Universidad de La Laguna, Tenerife (Spain); Lopez-Moreno, Sinhue [Escuela Superior Cd. Sahagun, Universidad Autonoma del Estado de Hidalgo, Carretera Cd. Sahagun-Otumba s/n. 43990, Hidalgo (Mexico); Humberto Romero, Aldo [Physics Department, West Virginia University, Morgantown, West Virginia 26506-6315 (United States); Max Planck Institut fuer Mikrostruktur Physik, Weinberg 2, 06120 Halle (Germany); Porcher, Florence; Andre, Gilles [Laboratoire Leon Brillouin, UMR12 CEA-CNRS, Bat 563 CEA Saclay, 91191 Gif sur Yvette Cedex (France); Poettgen, Rainer [Institut fuer Anorganische und Analytische Chemie, Universitaet Muenster, Corrensstrasse 30, 48149 Muenster (Germany)
2013-09-15
Within the series of ternary rare-earth transition metal carbides Sc{sub 3}TC{sub 4} (T = Fe, Co, Ni) only the Co congener displays a structural phase transition at 72 K and an onset of bulk superconductivity at 4.5 K. In this paper we present the results of a detailed analysis of the structural, electronic, and vibrational properties of the low-temperature phase of Sc{sub 3}CoC{sub 4} that represents one of the few well-documented examples of a quasi one-dimensional (1D) superconductor. Variable temperature neutron powder diffraction and low temperature X-ray diffraction experiments were performed in order to confirm the subtle structural distortions during the phase transition. The results of periodic electronic structure calculations indicate, that the structural transition can clearly be identified as a Peierls-type distortion and by a comparison with the isostructural carbide Sc{sub 3}FeC{sub 4} we are able to identify the chemical, electronic, and the vibrational control parameters of the transition. Topological analyses of the electron density distribution and of the valence shell charge concentrations at the cobalt atom finally allow us to directly correlate the changes in the electronic structure due to the Peierls transition in reciprocal space with the according subtle changes in the real space properties of Sc{sub 3}CoC{sub 4}. (Copyright copyright 2013 WILEY-VCH Verlag GmbH and Co. KGaA, Weinheim)
Ochi, Masayuki; Usui, Hidetomo; Kuroki, Kazuhiko
2017-12-01
Thermoelectric power generation has been recognized as one of the most important technologies, and high-performance thermoelectric materials have long been pursued. However, because of the large number of candidate materials, this quest is extremely challenging, and it has become clear that a firm theoretical concept from the viewpoint of band-structure engineering is needed. We theoretically demonstrate that pnictogen dichalcogenide layered compounds, which originally attracted attention as a family of superconductors and have recently been investigated as thermoelectric materials, can exhibit very high thermoelectric performance with elemental substitution. Specifically, we clarify a promising guiding principle for material design and find that LaOAsSe2, a material that has yet to be synthesized, has a power factor that is 6 times as large as that of the known compound LaOBiS2 and can exhibit a very large Z T under some plausible assumptions. This large enhancement of the thermoelectric performance originates from the quasi-one-dimensional gapped Dirac-like band dispersion, which is realized by the square-lattice network. We offer one ideal limit of the band structure for thermoelectric materials. Because our target materials have high controllability of constituent elements and feasibility of carrier doping, experimental studies along this line are eagerly awaited.
He, Mingquan; Wong, Chi Ho; Shi, Dian; Tse, Pok Lam; Scheidt, Ernst-Wilhelm; Eickerling, Georg; Scherer, Wolfgang; Sheng, Ping; Lortz, Rolf
2015-02-25
The transition metal carbide superconductor Sc(3)CoC(4) may represent a new benchmark system of quasi-one-dimensional (quasi-1D) superconducting behavior. We investigate the superconducting transition of a high-quality single crystalline sample by electrical transport experiments. Our data show that the superconductor goes through a complex dimensional crossover below the onset T(c) of 4.5 K. First, a quasi-1D fluctuating superconducting state with finite resistance forms in the [CoC(4)](∞) ribbons which are embedded in a Sc matrix in this material. At lower temperature, the transversal Josephson or proximity coupling of neighboring ribbons establishes a 3D bulk superconducting state. This dimensional crossover is very similar to Tl(2)Mo(6)Se(6), which for a long time has been regarded as the most appropriate model system of a quasi-1D superconductor. Sc(3)CoC(4) appears to be even more in the 1D limit than Tl(2)Mo(6)Se(6).
Xu, Xiaofeng; Jiao, W H; Zhou, N; Guo, Y; Li, Y K; Dai, Jianhui; Lin, Z Q; Liu, Y J; Zhu, Zengwei; Lu, Xin; Yuan, H Q; Cao, Guanghan
2015-08-26
We report on the quasi-linear in field intrachain magnetoresistance in the normal state of a quasi-one-dimensional superconductor Ta4Pd3Te16 (Tc ~ 4.6 K). Both the longitudinal and transverse in-chain magnetoresistance shows a power-law dependence, Δρ∝B(α) with the exponent α close to 1 over a wide temperature and field range. The magnetoresistance shows no sign of saturation up to 50 T studied. The linear magnetoresistance observed in Ta4Pd3Te16 is found to be overall inconsistent with the interpretations based on the Dirac fermions in the quantum limit, charge conductivity fluctuations as well as quantum electron-electron interference. Moreover, it is observed that the Kohler's rule, regardless of the field orientations, is violated in its normal state. This result suggests the loss of charge carriers in the normal state of this chain-containing compound, due presumably to the charge-density-wave fluctuations.
Chen, Chunlin; Yin, Deqiang; Inoue, Kazutoshi; Lichtenberg, Frank; Ma, Xiuliang; Ikuhara, Yuichi; Bednorz, Johannes Georg
2017-12-26
The quasi-one-dimensional (1D) metallic conductivity of the perovskite-related Sr n Nb n O 3n+2 compounds is of continuing fundamental physical interest as well as being important for developing advanced electronic devices. The Sr n Nb n O 3n+2 compounds can be derived by introducing additional oxygen into the SrNbO 3 perovskite. However, the physical origin for the transition of electrical properties from the three-dimensional (3D) isotropic conductivity in SrNbO 3 to the quasi-1D metallic conductivity in Sr n Nb n O 3n+2 requires more in-depth clarification. Here we combine advanced transmission electron microscopy with atomistic first-principles calculations to unambiguously determine the atomic and electronic structures of the Sr n Nb n O 3n+2 compounds and reveal the underlying mechanism for their quasi-1D metallic conductivity. We demonstrate that the local electrical conductivity in the Sr n Nb n O 3n+2 compounds directly depends on the configuration of the NbO 6 octahedra in local regions. These findings will shed light on the realization of two-dimensional (2D) electrical conductivity from a bulk material, namely by segmenting a 3D conductor into a stack of 2D conducting thin layers.
Neutron-scattering studies of the S=2 antiferromagnetic chain MnCl3(C10D8N2)
International Nuclear Information System (INIS)
Granroth, G.E.; Nagler, S.E.; Coldea, R.; Eccleston, R.S.; Ward, B.H.; Talham, D.R.; Meisel, M.W.
2002-01-01
Quasi-elastic and inelastic neutron scattering studies of the quasi-one-dimensional S=2 antiferromagnet MnCl 3 (C 10 D 8 N 2 ) are reported. The quasi-elastic measurements exhibit a broad peak at Q∼0.69 A -1 , which is consistent with short-range antiferromagnetic coupling between neighboring Mn 3+ ions. Inelastic experiments, at 150 mK and Q=0.70 A -1 , reveal decreased magnetic scattering at energies less than 0.2 meV when compared to similar studies at 20 K. These results provide microscopic evidence for the presence of a Haldane gap and are consistent with the bulk magnetization measurements of Granroth et al. (orig.)
International Nuclear Information System (INIS)
Freiberg, Arvi; Raetsep, Margus; Timpmann, Kou; Trinkunas, Gediminas
2009-01-01
Spectral characteristics of the optically excited states in the ring-shaped quasi-one-dimensional aggregates comprising 18 and 32 tightly coupled bacteriochlorophyll a molecules have been investigated using selective spectroscopy methods and theoretical modelling of the data. Distinguished by the lowest electronic transition energies in the LH2 and LH1 antenna complexes these aggregates govern the functionally important ultrafast funneling of solar excitation energy in the photosynthetic membranes of purple bacteria. It was found by using a sophisticated differential fluorescence line narrowing method that exciton-phonon coupling in terms of the dimensionless Huang-Rhys factor is strong in these systems, justifying an excitonic polaron theoretical approach for the data analysis. Although we reached this qualitative conclusion already previously, in this work essential dependence of the exciton-phonon coupling strength and reorganization energy on excitation wavelength as well as on excitation light fluence has been established. We then show that these results corroborate with the properties of excitonic polarons in diagonally disordered ensembles of the aggregates. Furthermore, the weighted density of states of the phonon modes, which is an important characteristic of dynamical systems interacting with their surroundings, was derived. Its shape, being similar for all studied circular aggregates, deviates significantly from a reference profile describing local response of a protein to the Q y electronic transition in a single bacteriochlorophyll a molecule. Similarities of the data for regular and B800 deficient mutant LH2 complexes indicate that the B800 pigments have no direct influence on the electronic states of the B850 aggregate system. Consistent set of model parameters was determined, unambiguously implying that excitonic polarons, rather than bare excitons are proper lowest-energy optical excitations in the LH1 and LH2 antenna complexes
Energy Technology Data Exchange (ETDEWEB)
Freiberg, Arvi [Institute of Physics, University of Tartu, Riia 142, 51014 Tartu (Estonia); Institute of Molecular and Cell Biology, University of Tartu, Riia 23, 51010 Tartu (Estonia)], E-mail: arvi.freiberg@ut.ee; Raetsep, Margus; Timpmann, Kou [Institute of Physics, University of Tartu, Riia 142, 51014 Tartu (Estonia); Trinkunas, Gediminas [Insitute of Physics, Savanoriu pr. 231, LT-02300 Vilnius (Lithuania)
2009-02-23
Spectral characteristics of the optically excited states in the ring-shaped quasi-one-dimensional aggregates comprising 18 and 32 tightly coupled bacteriochlorophyll a molecules have been investigated using selective spectroscopy methods and theoretical modelling of the data. Distinguished by the lowest electronic transition energies in the LH2 and LH1 antenna complexes these aggregates govern the functionally important ultrafast funneling of solar excitation energy in the photosynthetic membranes of purple bacteria. It was found by using a sophisticated differential fluorescence line narrowing method that exciton-phonon coupling in terms of the dimensionless Huang-Rhys factor is strong in these systems, justifying an excitonic polaron theoretical approach for the data analysis. Although we reached this qualitative conclusion already previously, in this work essential dependence of the exciton-phonon coupling strength and reorganization energy on excitation wavelength as well as on excitation light fluence has been established. We then show that these results corroborate with the properties of excitonic polarons in diagonally disordered ensembles of the aggregates. Furthermore, the weighted density of states of the phonon modes, which is an important characteristic of dynamical systems interacting with their surroundings, was derived. Its shape, being similar for all studied circular aggregates, deviates significantly from a reference profile describing local response of a protein to the Q{sub y} electronic transition in a single bacteriochlorophyll a molecule. Similarities of the data for regular and B800 deficient mutant LH2 complexes indicate that the B800 pigments have no direct influence on the electronic states of the B850 aggregate system. Consistent set of model parameters was determined, unambiguously implying that excitonic polarons, rather than bare excitons are proper lowest-energy optical excitations in the LH1 and LH2 antenna complexes.
Energy Technology Data Exchange (ETDEWEB)
Langie da Silva, Douglas, E-mail: douglas.langie@ufpel.edu.br [Departamento de Física, Universidade Federal de Pelotas, Caixa Postal 354, Pelotas 96010-900 (Brazil); Moreira, Eduardo Ceretta [Laboratório de Espectroscopia, Universidade Federal do Pampa, Campus Bagé, Bagé 96400-970 (Brazil); Dias, Fábio Teixeira; Neves Vieira, Valdemar das [Departamento de Física, Universidade Federal de Pelotas, Caixa Postal 354, Pelotas 96010-900 (Brazil); Brandt, Iuri Stefani; Cas Viegas, Alexandre da; Pasa, André Avelino [Laboratório de Filmes Finos e Superfícies, Universidade Federal de Santa Catarina, Caixa Postal 476, Florianópolis 88.040-900 (Brazil)
2015-01-15
Nanostructured cobalt vanadium oxide (V{sub 2}O{sub 5}) xerogels spread onto crystalline Si substrates were synthesized via peroxovanadate sol gel route. The resulting products were characterized by distinct experimental techniques. The surface morphology and the nanostructure of xerogels correlate with Co concentration. The decrease of the structural coherence length is followed by the formation of a loose network of nanopores when the concentration of intercalated species was greater than 4 at% of Co. The efficiency of the synthesis route also drops with the increase of Co concentration. The interaction between the Co(OH{sub 2}){sub 6}{sup 2+} cations and the (H{sub 2}V{sub 10}O{sub 28}){sup 4−} anions during the synthesis was suggested as a possible explanation for the incomplete condensation of the V{sub 2}O{sub 5} gel. Finally the experimental results points for the intercalation of Co between the bilayers of the V{sub 2}O{sub 5}. In this scenario two possible preferential occupation sites for the metallic atoms in the framework of the xerogel were proposed. - Graphical abstract: Quasi-one-dimensional nanostructured cobalt (Co) intercalated vanadium oxide (V{sub 2}O{sub 5}) nanoribbons synthesized by peroxovanadate sol gel route. - Highlights: • Nanostructured cobalt V{sub 2}O{sub 5} gel spread onto c{sub S}i were synthesized via peroxovanadate sol gel route. • The micro and nanostructure correlates with the cobalt content. • The efficiency of the synthesis route shows to be also dependent of Co content. • The experimental results points for the intercalation of Co between the bilayers of the V{sub 2}O{sub 5} xerogel.
Non-resonant precession of the neutron magnetic moment in antiferromagnets
International Nuclear Information System (INIS)
Skoblin, A.A.
1995-01-01
It is shown that the magnetic moment of a neutron moving in an antiferromagnet with a spiral-order magnetic field slowly precesses. Precession pitch strongly depends on the value and direction of the neutron velocity. 4 refs
Granroth, G E; Coldea, R; Eccleston, R S; Ward, B H; Talham, D R; Meisel, M W
2002-01-01
Quasi-elastic and inelastic neutron scattering studies of the quasi-one-dimensional S=2 antiferromagnet MnCl sub 3 (C sub 1 sub 0 D sub 8 N sub 2) are reported. The quasi-elastic measurements exhibit a broad peak at Q approx 0.69 A sup - sup 1 , which is consistent with short-range antiferromagnetic coupling between neighboring Mn sup 3 sup + ions. Inelastic experiments, at 150 mK and Q=0.70 A sup - sup 1 , reveal decreased magnetic scattering at energies less than 0.2 meV when compared to similar studies at 20 K. These results provide microscopic evidence for the presence of a Haldane gap and are consistent with the bulk magnetization measurements of Granroth et al. (orig.)
External magnetic field induced anomalies of spin nuclear dynamics in thin antiferromagnetic films
International Nuclear Information System (INIS)
Tarasenko, S.V.
1995-01-01
It is shown that if the thickness of homogeneously magnetized plate of high-axial antiferromagnetic within H external magnetic field becomes lower the critical one, then the effect of dynamic magnetoelastic interaction on Soul-Nakamura exchange of nuclear spins results in formation of qualitatively new types of spreading nuclear spin waves no else compared neither within the model of unrestricted magnetic nor at H = 0 in case of thin plate of high-axial antiferromagnetic. 10 refs
Magnetic and elastic properties of the antiferromagnet uranium mononitride
International Nuclear Information System (INIS)
Van Doorn, C.F.
1976-10-01
The magnetic and elastic properties of antiferromagnetic uranium mononitride single crystals are studied in the thesis from the measurements of the temperature dependences of the magnetic susceptibility, electrical resistivity and elastic constants. The elastic constants C 11 , C 12 and C 44 were determined in the temperature interval 4 to 300 K by ultrasonic measurements of the five possible wave velocities in the [100] and [110] directions. A test for internal consistency was also made. A dip of about 9 percent occurs in C 11 at a temperature of 5 to 6 K lower than the Neel temperature T(N) (equals about 53 K). Starting at T(N), a renormalization in C 44 is proportional to the square of the sublattice magnetization also occurs. Both these results agree with model calculations which include spin-phonon interactions. The investigation of this anomaly was extended by measuring the electrical resistivity of a sample cut from the same crystal as that on which the elasticity was measured. No anomalous behavior was observed at the temperature where C 11 displays its anomaly. However, a discontinuity in the temperature derivative of the resistance was found at T(N). The possible effect of a magnetic field on the resistivity, as well as on the elasticity, was investigated without any measurable effect. The magnetic susceptibility was measured with a Foner magnetometer between 4 and 1 000 K. It was found that above the Neel temperature the paramagnetic susceptibility followed a revised Curie-Weiss law. In an attempt to ascertain the ionic state of the 5f-uranium ion in UN, use was made of the experimentally determined Weiss constant, spin disorder resistivity and Knight shift. A calculation was made that gave a good representation of the ratio of the experimental susceptibilities along the [100] and [110] directions in the ordered region [af
International Nuclear Information System (INIS)
Zhao-Sen, Liu; Vladimir, Sechovský; Martin, Diviš
2011-01-01
A Usov-type quantum model based on a mean-field approximation is utilized to simulate the magnetic structure of an assumed rare-earth nanoparticle consisting of an antiferromagnetic core and a paramagnetic outer shell. We study the magnetic properties in the presence and absence of an external magnetic field. Our simulation results show that the magnetic moments in the core region orientate antiferromagnetically in zero external magnetic field; an applied magnetic field rotates all of the magnetic moments in the paramagnetic shell completely to the field direction, and turns those in the core (which tries to maintain its original antiferromagnetic structure) towards the orientation in some degree; and the paramagnetic shell does not have a strong influence on the magnetic configuration of the core. (condensed matter: electronic structure, electrical, magnetic, and optical properties)
Ignatenko, A. N.; Irkhin, V. Yu.
2016-01-01
We have studied the Heisenberg antiferromagnets characterized by the magnetic structures with the periods being two times larger than the lattice period. We have considered all the types of the Bravais lattices (simple cubic, bcc and fcc) and divided all these antiferromagnets into 7 classes i.e. 3 plus 4 classes denoted with symbols A and B correspondingly. The order parameter characterizing the degeneracies of the magnetic structures is an ordinary Neel vector for A classes and so-called 4-...
Energy Technology Data Exchange (ETDEWEB)
Bukharov, A A; Ovchinnikov, A S; Baranov, N V [Department of Physics, Ural State University, Ekaterinburg, 620083 (Russian Federation); Inoue, K [Institute for Advanced Materials Research, Hiroshima University, Hiroshima (Japan)
2010-11-03
Using Monte Carlo simulations we investigate magnetic hysteresis in two- and three-dimensional systems of weakly antiferromagnetically coupled spin chains based on a scenario of domain wall (kink) motion within the chains. By adapting the model of walkers to simulate the domain wall dynamics and using the Ising-like dipole-dipole model, we study the effects of interchain coupling, temperature and anisotropy axis direction on hysteresis curves.
Srivastava, P.; Chaudhary, S.; Maurya, V.; Saha, J.; Kaushik, S. D.; Siruguri, V.; Patnaik, S.
2018-05-01
Synthesis and extensive structural, pyroelectric, magnetic, dielectric and magneto-electric characterizations are reported for polycrystalline Co4Nb2O9 towards unraveling the multiferroic ground state. Magnetic measurements confirm that Co4Nb2O9 becomes an anti-ferromagnet at around 28 K. Associated with the magnetic phase transition, a sharp peak in pyroelectric current indicates the appearance of strong magneto-electric coupling below Neel temperature (TN) along with large coupling constant upto 17.8 μC/m2T. Using temperature oscillation technique, we establish Co4Nb2O9 to be a genuine multiferroic with spontaneous electric polarization in the anti-ferromagnetic state in the absence of magnetic field poling. This is in agreement with our low temperature neutron diffraction studies that show the magnetic structure of Co4Nb2O9 to be that of a non-collinear anti-ferromagnet with ferroelectric ground state.
Magnetic correlations in the intermetallic antiferromagnet Nd3Co4Sn13
Wang, C. W.; Lin, J. W.; Lue, C. S.; Liu, H. F.; Kuo, C. N.; Mole, R. A.; Gardner, J. S.
2017-11-01
Specific heat, magnetic susceptibility, and neutron scattering have been used to investigate the nature of the spin system in the antiferromagnet Nd3Co4Sn13. At room temperature Nd3Co4Sn13 has a cubic, Pm-3n structure similar to Yb3Rh4Sn13. Antiferromagnetic interactions between, Nd3+ ions dominate the magnetic character of this sample and at 2.4 K the Nd spins enter a long range order state with a magnetic propagation vector q = (0 0 0) with an ordered moment of 1.78(2) µ B at 1.5 K. The magnetic Bragg intensity grows very slowly below 1 K, reaching ~2.4 µ B at 350 mK. The average magnetic Nd3+ configuration corresponds to the 3D irreducible representation Γ7. This magnetic structure can be viewed as three sublattices of antiferromagnetic spin chains coupled with each other in the 120°-configuration. A well-defined magnetic excitation was measured around the 1 1 1 zone centre and the resulting dispersion curve is appropriate for an antiferromagnet with a gap of 0.20(1) meV.
DEFF Research Database (Denmark)
Larsen, J.; Schäffer, T. K.; Hansen, U. B.
2017-01-01
We present experimental evidence for a quantum phase transition in the easy-axis S = 3/2 anisotropic quasione-dimensional ferromagnet CoCl2 · 2D2O in a transverse field. Elastic neutron scattering shows that the magnetic order parameter vanishes at a transverse critical field μ0Hc = 16.05(4) T......, while inelastic neutron scattering shows that the gap in the magnetic excitation spectrum vanishes at the same field value, and reopens for H>Hc. The field dependence of the order parameter and the gap are well described by critical exponents β = 0.45 ± 0.09 and zν close to 1/2, implying...... that the quantum phase transition in CoCl2 · 2D2O differs significantly from the textbook version of a S = 1/2 Ising chain in a transverse field. We attribute the difference to weak but finite three-dimensionality of the magnetic interactions....
All-oxide-based synthetic antiferromagnets exhibiting layer-resolved magnetization reversal
Chen, Binbin; Xu, Haoran; Ma, Chao; Mattauch, Stefan; Lan, Da; Jin, Feng; Guo, Zhuang; Wan, Siyuan; Chen, Pingfan; Gao, Guanyin; Chen, Feng; Su, Yixi; Wu, Wenbin
2017-07-01
Synthesizing antiferromagnets with correlated oxides has been challenging, owing partly to the markedly degraded ferromagnetism of the magnetic layer at nanoscale thicknesses. Here we report on the engineering of an antiferromagnetic interlayer exchange coupling (AF-IEC) between ultrathin but ferromagnetic La2/3Ca1/3MnO3 layers across an insulating CaRu1/2Ti1/2O3 spacer. The layer-resolved magnetic switching leads to sharp steplike hysteresis loops with magnetization plateaus depending on the repetition number of the stacking bilayers. The magnetization configurations can be switched at moderate fields of hundreds of oersted. Moreover, the AF-IEC can also be realized with an alternative magnetic layer of La2/3Sr1/3MnO3 that possesses a Curie temperature near room temperature. The findings will add functionalities to devices with correlated-oxide interfaces.
Extended quantum critical phase in a magnetized spin-1/2 antiferromagnetic chain
DEFF Research Database (Denmark)
Stone, M.B.; Reich, D.H.; Broholm, C.
2003-01-01
Measurements are reported of the magnetic field dependence of excitations in the quantum critical state of the spin S=1/2 linear chain Heisenberg antiferromagnet copper pyrazine dinitrate (CuPzN). The complete spectrum was measured at k(B)T/Jless than or equal to0.025 for H=0 and H=8.7 T, where...
Onoda, M
2003-01-01
The structural and electronic properties of the Li sub 1 sub + sub x V sub 3 O sub 8 insertion electrode, where 0 sup 0.1 with nearly stoichiometric oxygen atoms, small polarons exist without carrier-creation energy at high temperatures, while at low temperatures the conduction may be of variable-range hopping (VRH) type. For x > 0.2, one-dimensional magnetic properties appear due to sizable exchange couplings and order-disorder effects of additional Li ions may lead to significant change of transport properties. For the intermediate composition 0 < x sup<= 0.1, strong randomness of the Li doping and the congenital oxygen deficiency cause VRH states even at high temperatures.
Aizawa, Hirohito; Kuroki, Kazuhiko
2018-03-01
We present a first-principles band calculation for the quasi-one-dimensional (Q1D) organic superconductor (TMTSF) 2ClO4 . An effective tight-binding model with the TMTSF molecule to be regarded as the site is derived from a calculation based on maximally localized Wannier orbitals. We apply a two-particle self-consistent (TPSC) analysis by using a four-site Hubbard model, which is composed of the tight-binding model and an onsite (intramolecular) repulsive interaction, which serves as a variable parameter. We assume that the pairing mechanism is mediated by the spin fluctuation, and the sign of the superconducting gap changes between the inner and outer Fermi surfaces, which correspond to a d -wave gap function in a simplified Q1D model. With the parameters we adopt, the critical temperature for superconductivity estimated by the TPSC approach is approximately 1 K, which is consistent with experiment.
Magnetic properties of the strongly correlated chain antiferromagnet KTb(WO4)2
International Nuclear Information System (INIS)
Khatsko, E.; Loginov, A.; Cherny, A.; Rykova, A.
2006-01-01
The susceptibility and magnetization of a single crystal of KTb(WO 4 ) 2 has been measured in the temperature range 0.5-80 K in magnetic fields up to 6 T. It is shown that KTb(WO 4 ) 2 is an Ising magnet with only one component of the magnetic moment. The three-dimensional phase transition to the antiferromagnetically ordered state has been found below 0.7 K. This transition can be described in the molecular field two-level approximation. The principal exchange constant has been estimated. By using experimental data the magnetic structure of KTb(WO 4 ) 2 is proposed
Magnetic Anisotropy by Rashba Spin-Orbit Coupling in Antiferromagnetic Thin Films
Ieda, Jun'ichi; Barnes, Stewart E.; Maekawa, Sadamichi
2018-05-01
Magnetic anisotropy in an antiferromagnet (AFM) with inversion symmetry breaking (ISB) is investigated. The magnetic anisotropy energy (MAE) resulting from the Rashba spin-orbit and s-d type exchange interactions is determined for two different models of AFMs. The global ISB model, representing the effect of a surface, an interface, or a gating electric field, results in an easy-plane magnetic anisotropy. In contrast, for a local ISB model, i.e., for a noncentrosymmetric AFM, perpendicular magnetic anisotropy (PMA) arises. Both results differ from the ferromagnetic case, in which the result for PMA depends on the band structure and dimensionality. These MAE contributions play a key role in determining the direction of the Néel order parameter in antiferromagnetic nanostructures, and reflect the possibility of electrical-field control of the Néel vector.
Magnetization process in antiferromagnetic EuPdIn
International Nuclear Information System (INIS)
Ito, T.; Nishigori, S.; Hiromitsu, I.
1998-01-01
Magnetization and magnetic susceptibility measurements have been m[e on EuPdIn single crystals. Isothermal magnetization curves measured along the a-, b- and c-axis exhibit three anomalies at the maximum. The phase diagrams determined by the critical fields are explained by the molecular field theory in weak magnetocrystalline anisotropy. (orig.)
Nonlocally sensing the magnetic states of nanoscale antiferromagnets with an atomic spin sensor.
Yan, Shichao; Malavolti, Luigi; Burgess, Jacob A J; Droghetti, Andrea; Rubio, Angel; Loth, Sebastian
2017-05-01
The ability to sense the magnetic state of individual magnetic nano-objects is a key capability for powerful applications ranging from readout of ultradense magnetic memory to the measurement of spins in complex structures with nanometer precision. Magnetic nano-objects require extremely sensitive sensors and detection methods. We create an atomic spin sensor consisting of three Fe atoms and show that it can detect nanoscale antiferromagnets through minute, surface-mediated magnetic interaction. Coupling, even to an object with no net spin and having vanishing dipolar stray field, modifies the transition matrix element between two spin states of the Fe atom-based spin sensor that changes the sensor's spin relaxation time. The sensor can detect nanoscale antiferromagnets at up to a 3-nm distance and achieves an energy resolution of 10 μeV, surpassing the thermal limit of conventional scanning probe spectroscopy. This scheme permits simultaneous sensing of multiple antiferromagnets with a single-spin sensor integrated onto the surface.
Nonlocally sensing the magnetic states of nanoscale antiferromagnets with an atomic spin sensor
Yan, Shichao; Malavolti, Luigi; Burgess, Jacob A. J.; Droghetti, Andrea; Rubio, Angel; Loth, Sebastian
2017-01-01
The ability to sense the magnetic state of individual magnetic nano-objects is a key capability for powerful applications ranging from readout of ultradense magnetic memory to the measurement of spins in complex structures with nanometer precision. Magnetic nano-objects require extremely sensitive sensors and detection methods. We create an atomic spin sensor consisting of three Fe atoms and show that it can detect nanoscale antiferromagnets through minute, surface-mediated magnetic interaction. Coupling, even to an object with no net spin and having vanishing dipolar stray field, modifies the transition matrix element between two spin states of the Fe atom–based spin sensor that changes the sensor’s spin relaxation time. The sensor can detect nanoscale antiferromagnets at up to a 3-nm distance and achieves an energy resolution of 10 μeV, surpassing the thermal limit of conventional scanning probe spectroscopy. This scheme permits simultaneous sensing of multiple antiferromagnets with a single-spin sensor integrated onto the surface. PMID:28560346
QUASI-ONE DIMENSIONAL CLASSICAL FLUIDS
Directory of Open Access Journals (Sweden)
J.K.Percus
2003-01-01
Full Text Available We study the equilibrium statistical mechanics of simple fluids in narrow pores. A systematic expansion is made about a one-dimensional limit of this system. It starts with a density functional, constructed from projected densities, which depends upon projected one and two-body potentials. The nature of higher order corrections is discussed.
International Nuclear Information System (INIS)
Fukushima, Akio; Yakushiji, Kay; Konoto, Makoto; Kubota, Hitoshi; Imamura, Hiroshi; Yuasa, Shinji
2016-01-01
We newly developed a magnetic memory cell having multi-bit function. The memory cell composed of a perpendicularly magnetized magnetic tunnel junction (MB-pMTJ) and a synthetic antiferromagnetic reference layer. The multi-bit function is realized by combining the freedom of states of the magnetic free layer and that in the antiferromagnetically coupled reference layer. The structure of the reference layer is (FeB/Ta/[Co/Pt]_3)/Ru/([Co/Pt]_6); the top and the bottom layers are coupled through Ru layer where the reference layer has two degrees of freedom of a head-to-head and a bottom-to-bottom magnetic configuration. A four-state memory cell is realized by combination of both degrees of freedom. The states in the reference layer however is hardly detected by the total resistance of MB-pMTJ, because the magnetoresistance effect in the reference layer is negligibly small. That implies that the resistance values for the different states in the reference layer are degenerated. On the other hand, the two different states in the reference layer bring different stray fields to the free layer, which generate two different minor loop with different switching fields. Therefore, the magnetic states in the reference layer can be differentiated by the two-step reading, before and after applying the appropriately pulsed magnetic field which can identify the initial state in the reference layer. This method is similar to distinguishing different magnetic states in an in-plane magnetized spin-valve element. We demonstrated that four different states in the MB-pMTJ can be distinguished by the two-step read-out. The important feature of the two-step reading is a practically large operation margins (large resistance change in reading) which is equal to that of a single MTJ. Even though the two-step reading is a destructive method by which 50% of the magnetic state is changed, this MB-pMTJ is promising for high density non-volatile memory cell with a minor cost of operation speed
Neutron diffraction study of antiferromagnetic ErNi3Ga9 in magnetic fields
Ninomiya, Hiroki; Sato, Takaaki; Matsumoto, Yuji; Moyoshi, Taketo; Nakao, Akiko; Ohishi, Kazuki; Kousaka, Yusuke; Akimitsu, Jun; Inoue, Katsuya; Ohara, Shigeo
2018-05-01
We report specific heat, magnetization, magnetoresistance, and neutron diffraction measurements of single crystals of ErNi3Ga9. This compound crystalizes in a chiral structure with space group R 32 . The erbium ions form a two-dimensional honeycomb structure. ErNi3Ga9 displays antiferromagnetic order below 6.4 K. We determined that the magnetic structure is slightly amplitude-modulated as well as antiferromagnetic with q = (0 , 0 , 0.5) . The magnetic properties are described by an Ising-like model in which the magnetic moment is always along the c-axis owing to the large uniaxial anisotropy caused by the crystalline electric field effect in the low temperature region. When the magnetic field is applied along the c-axis, a metamagnetic transition is observed around 12 kOe at 2 K. ErNi3Ga9 possesses crystal chirality, but the antisymmetric magnetic interaction, the so-called Dzyaloshinskii-Moriya (DM) interaction, does not contribute to the magnetic structure, because the magnetic moments are parallel to the DM-vector.
Institute of Scientific and Technical Information of China (English)
段玲; 胡飞; 丁建文
2011-01-01
考虑实际体系的梯度无序和结散射,发展格林函数矩阵分解消元方法,研究了准一维纳米线的电子输运性质.结果表明,由于结散射,电导随能量呈现振荡行为,无序的引入破坏了电子相干性,在低无序度区平均电导呈现异常增加,呈现一个新的电导峰.当表面存在无序但无梯度衰减时,体系的平均电导随无序度增强先减后增,出现类局域—退局域性转变.当表面无序线性衰减时,平均电导在强无序区稍有增加,而当表面无序高斯型衰减时,平均电导指数衰减,类局域—退局域性转变消失,不同于以前的理论预言.研究结果对准一维纳米线电子器件的结构设计和应用有指导作用.%Considering both the gradient decay of the real disorder and the contact scattering,we investigate the electronic transport in quasi-one-dimensional nanowires by developing a decomposition elimination method for Green＇s function matrix.In the presence the contact scattering,the conductance oscillates with energy.For some energies of incident electrons,an abnormal enhancement is obtained in the average conductance due to the destroyed coherence by the introduction of much low disorder,showing that there appears a new conductance peak.In the absence of disorder gradient,the average conductance firstly decreases then increases with disorder strength,indicating that there exists a localization-delocalization transition.In the presence of linearly decaying disorder,the average conductance increases slightly in a strong disorder region.In the case of the Gaussian-type decaying disorder,the average conductance decreases exponentially and the localization-delocalization transition disappears,which is different from previous thereotical result.The results are helpful for the design and the application of quasi-one-dimensional nanowires device.
Small clusters with anisotropic antiferromagnetic exchange in a magnetic field
International Nuclear Information System (INIS)
Parkinson, J B; Elliott, R J; Timonen, J
2004-01-01
We consider small symmetric clusters of magnetic atoms (spins) with anisotropic exchange interaction between the atoms in a magnetic field at zero temperature. The inclusion of the anisotropy leads to a wealth of different phases as a function of the applied magnetic field. These are not phases in the thermodynamic sense with critical properties but rather physical structures with different arrangements of the spins and hence different symmetries. We study the spatial symmetry of these phases, for the classical and quantum cases. Results are presented mainly for three frustrated systems, the triangle, the tetrahedron and the five-atom ring, which have many interesting features. In the classical limit we obtain phase diagrams in which some of the phase changes occur because of energy crossings and others due to energy bifurcations, corresponding to 'first-' and 'second-order' changes. In the quantum case we show how the symmetries of the states are related to the corresponding classical symmetries
Novel magnetic hydrogen sensing: a case study using antiferromagnetic haematite nanoparticles
International Nuclear Information System (INIS)
Punnoose, Alex; Reddy, K M; Thurber, Aaron; Hays, Jason; Engelhard, Mark H
2007-01-01
Hydrogen sensing is a critical component of safety to address widespread public perceptions of the hazards of production, storage, transportation and use of hydrogen in proposed future automobiles and in various other applications. A nanoscale magnetic hydrogen sensor is proposed based on the experimental observation of systematically varying the saturation magnetization and remanence of nanoscale antiferromagnetic haematite with hydrogen flow. The saturation magnetization and remanence of the nanoscale haematite sample showed an increase of one to two orders of magnitude in the presence of flowing hydrogen gas at concentrations in the 1-10% range and at 575 K, suggesting that a practical magnetic hydrogen sensor could be developed using this material and the novel magnetic sensing method. Thermogravimetric analysis of the haematite sample shows significant mass loss when hydrogen gas is introduced. X-ray diffraction and x-ray photoelectron spectroscopy studies ruled out any impurity phase formation as a result of gas-sample interaction. This work thus facilitates the use of the magnetic properties of an antiferromagnetic material as gas sensing parameters, thus exploring the concept of 'magnetic gas sensing'
Baltz, V.; Manchon, A.; Tsoi, M.; Moriyama, T.; Ono, T.; Tserkovnyak, Y.
2018-01-01
Antiferromagnetic materials could represent the future of spintronic applications thanks to the numerous interesting features they combine: they are robust against perturbation due to magnetic fields, produce no stray fields, display ultrafast dynamics, and are capable of generating large magnetotransport effects. Intense research efforts over the past decade have been invested in unraveling spin transport properties in antiferromagnetic materials. Whether spin transport can be used to drive the antiferromagnetic order and how subsequent variations can be detected are some of the thrilling challenges currently being addressed. Antiferromagnetic spintronics started out with studies on spin transfer and has undergone a definite revival in the last few years with the publication of pioneering articles on the use of spin-orbit interactions in antiferromagnets. This paradigm shift offers possibilities for radically new concepts for spin manipulation in electronics. Central to these endeavors are the need for predictive models, relevant disruptive materials, and new experimental designs. This paper reviews the most prominent spintronic effects described based on theoretical and experimental analysis of antiferromagnetic materials. It also details some of the remaining bottlenecks and suggests possible avenues for future research. This review covers both spin-transfer-related effects, such as spin-transfer torque, spin penetration length, domain-wall motion, and "magnetization" dynamics, and spin-orbit related phenomena, such as (tunnel) anisotropic magnetoresistance, spin Hall, and inverse spin galvanic effects. Effects related to spin caloritronics, such as the spin Seebeck effect, are linked to the transport of magnons in antiferromagnets. The propagation of spin waves and spin superfluids in antiferromagnets is also covered.
Talantsev, A.; Lu, Y.; Fache, T.; Lavanant, M.; Hamadeh, A.; Aristov, A.; Koplak, O.; Morgunov, R.; Mangin, S.
2018-04-01
Two synthetic antiferromagnet bilayer systems with strong perpendicular anisotropy CoFeB/Ta/CoFeB and Pt/Co/Ir/Co/Pt have been grown using sputtering techniques. For both systems two types of magnetization transitions have been studied. The first one concerns transitions from a state where magnetizations of the two magnetic layers are parallel (P state) to a state where magnetizations of the two layers are aligned antiparallel (AP state). The second one concerns transitions between the two possible antiparallel alignments (AP+ to AP-). For both systems and both transitions after-effect measurements can be understood in the frame of nucleation—propagation model. Time derivative analysis of magnetic relaxation curves and mapping of the first order reversal curves at different temperature allowed us to demonstrate the presence of different pinning centers, which number can be controlled by magnetic field and temperature.
Narrow and broad solitons in the antiferromagnetic chains of CsCoCl3 and TMMC
International Nuclear Information System (INIS)
Boucher, J.P.; Regnault, L.P.; Pires, A.; Rossat-Mignod, J.; Henry, Y.; Bouillot, J.; Stirling, W.G.; Renard, J.P.
1984-06-01
The two quasi one-dimensional (1D) compounds CsCoCl 3 and (CH 3 ) 4 NMnCl 3 (TMMC) are almost ideal systems in which to study soliton excitations. Both they have antiferromagnetic (AF) couplings in the chains and at low temperature they exhibit an Ising symmetry favourable for the occurence of solitons. This symmetry is an intrinsic property of CsCoCl 3 while in TMMC it is only achieved by the application of an external magnetic field H perpendicular to the chains. In the lD short range order regime two energetically equivalent configurations are expected for the spins. Solitons can be seen as Bloch walls separating ordered domains and allowing the spins to pass from one configuration to the other. In the case of a ''strong'' Ising symmetry (CsCoCl 3 ) the walls are reduced to one lattice unit (''narrow'' solitons) while in the case of a ''weak'' Ising symmetry (TMMC) the walls extend over several lattice units (10 to 30) (''broad'' solitons). To maintain a paramagnetic state, these walls move rapidly along the chains inducing characteristic fluctuations. The investigation of these two compounds, CsCoCl 3 and TMMC illustrates the advantage of antiferromagnets as the AF mode yields an accurate determination of the soliton regime. Narrow and broad solitons are observed to behave very similarly
International Nuclear Information System (INIS)
Martinez, E.; Vega, A.; Robles, R.; Vazquez de Parga, A.L.
2005-01-01
We present a theoretical study of the magnetic properties of thin Mn films of 6 and 7 monolayers supported on Fe(001). The ab-initio tight binding linear muffin tin orbital (TB-LMTO) method was used to investigate the competition between ferromagnetic (F) and antiferromagnetic (AF) couplings within the system. We found several collinear magnetic solutions that may coexist at room temperature. The most stable configurations are characterized by AF coupling between the surface and subsurface Mn layers together with F coupling between Mn and Fe at the interface. The ground state arrangements for the 6 and 7 Mn films display opposite sign of the surface magnetic moment relative to the Fe substrate. The implications of these results in the possible onset of non-collinear magnetism when a step is present at the interface are discussed in comparison with Cr/Fe systems where non-collinear magnetism has been recently reported
Baltz, V.; Manchon, Aurelien; Tsoi, M.; Moriyama, T.; Ono, T.; Tserkovnyak, Y.
2018-01-01
Antiferromagnetic materials could represent the future of spintronic applications thanks to the numerous interesting features they combine: they are robust against perturbation due to magnetic fields, produce no stray fields, display ultrafast dynamics, and are capable of generating large magnetotransport effects. Intense research efforts over the past decade have been invested in unraveling spin transport properties in antiferromagnetic materials. Whether spin transport can be used to drive the antiferromagnetic order and how subsequent variations can be detected are some of the thrilling challenges currently being addressed. Antiferromagnetic spintronics started out with studies on spin transfer and has undergone a definite revival in the last few years with the publication of pioneering articles on the use of spin-orbit interactions in antiferromagnets. This paradigm shift offers possibilities for radically new concepts for spin manipulation in electronics. Central to these endeavors are the need for predictive models, relevant disruptive materials, and new experimental designs. This paper reviews the most prominent spintronic effects described based on theoretical and experimental analysis of antiferromagnetic materials. It also details some of the remaining bottlenecks and suggests possible avenues for future research. This review covers both spin-transfer-related effects, such as spin-transfer torque, spin penetration length, domain-wall motion, and
Baltz, V.
2018-02-15
Antiferromagnetic materials could represent the future of spintronic applications thanks to the numerous interesting features they combine: they are robust against perturbation due to magnetic fields, produce no stray fields, display ultrafast dynamics, and are capable of generating large magnetotransport effects. Intense research efforts over the past decade have been invested in unraveling spin transport properties in antiferromagnetic materials. Whether spin transport can be used to drive the antiferromagnetic order and how subsequent variations can be detected are some of the thrilling challenges currently being addressed. Antiferromagnetic spintronics started out with studies on spin transfer and has undergone a definite revival in the last few years with the publication of pioneering articles on the use of spin-orbit interactions in antiferromagnets. This paradigm shift offers possibilities for radically new concepts for spin manipulation in electronics. Central to these endeavors are the need for predictive models, relevant disruptive materials, and new experimental designs. This paper reviews the most prominent spintronic effects described based on theoretical and experimental analysis of antiferromagnetic materials. It also details some of the remaining bottlenecks and suggests possible avenues for future research. This review covers both spin-transfer-related effects, such as spin-transfer torque, spin penetration length, domain-wall motion, and
Magnetic response of hybrid ferromagnetic and antiferromagnetic core-shell nanostructures.
Khan, U; Li, W J; Adeela, N; Irfan, M; Javed, K; Wan, C H; Riaz, S; Han, X F
2016-03-21
The synthesis of FeTiO3-Ni(Ni80Fe20) core-shell nanostructures by a two-step method (sol-gel and DC electrodeposition) has been demonstrated. XRD analysis confirms the rhombohedral crystal structure of FeTiO3(FTO) with space group R3[combining macron]. Transmission electron microscopy clearly depicts better morphology of nanostructures with shell thicknesses of ∼25 nm. Room temperature magnetic measurements showed significant enhancement of magnetic anisotropy for the permalloy (Ni80Fe20)-FTO over Ni-FTO core-shell nanostructures. Low temperature magnetic measurements of permalloy-FeTiO3 core-shell structure indicated a strong exchange bias mechanism with magnetic coercivity below the antiferromagnetic Neel temperature (TN = 59 K). The exchange bias is attributed to the alignment of magnetic moments in the antiferromagnetic material at low temperature. Our scheme opens a path towards optimum automotive systems and wireless communications wherein broader bandwidths and smaller sizes are required.
International Nuclear Information System (INIS)
Cui Yan; Li Yan-Rong; Li Rui-Yuan; Wang Yun-Ping
2014-01-01
We perform both dc and ac magnetic measurements on the single crystal of Mn 3 O(Et-sao) 3 (ClO 4 )(MeOH) 3 single-molecule magnet (SMM) when the sample is preserved in air for different durations. We find that, during the oxidation process, the sample develops into another SMM with a smaller anisotropy energy barrier and a stronger antiferromagnetic intermolecular exchange interaction. The antiferromagnetic transition temperature observed at 6.65 K in the new SMM is record-high for the antiferromagnetic phase transition in all the known SMMs. Compared to the original SMM, the only apparent change for the new SMM is that each molecule has lost three methyl groups as revealed by four-circle x-ray diffraction (XRD), which is thought to be the origin of the stronger antiferromagnetic intermolecular exchange interaction
International Nuclear Information System (INIS)
Okamoto, J.; Mamiya, K.; Fujimori, S.-I.; Okane, T.; Saitoh, Y.; Muramatsu, Y.; Fujimori, A.; Ishiwata, S.; Takano, M.
2004-01-01
Magnetic circular x-ray dichroism (MCXD) measurements in Fe 2p absorption have been done on SrFeO3, which shows a spiral anti-ferromagnetism, by using a 10-T superconducting magnet. Finite MCXD structures have been observed under magnetic field of 8 T even in the paramagnetic and anti-ferromagnetic states. The intensity of the MCXD structure at hv ∼ 710 eV increases linearly as magnetic field increases linearly and the total magnetic moments estimated by MCXD sum rules roughly corresponds to the magnetization measured by SQUID measurements. MCXD study of paramagnetic and/or anti-ferromagnetic samples can be done by using a superconducting magnet that generates a strong magnetic field enough to induce finite magnetization
Perspectives of antiferromagnetic spintronics
Jungfleisch, Matthias B.; Zhang, Wei; Hoffmann, Axel
2018-04-01
Antiferromagnets are promising for future spintronic applications owing to their advantageous properties: They are magnetically ordered, but neighboring magnetic moments point in opposite directions, which results in zero net magnetization. This means antiferromagnets produce no stray fields and are insensitive to external magnetic field perturbations. Furthermore, they show intrinsic high frequency dynamics, exhibit considerable spin-orbit and magneto-transport effects. Over the past decade, it has been realized that antiferromagnets have more to offer than just being utilized as passive components in exchange bias applications. This development resulted in a paradigm shift, which opens the pathway to novel concepts using antiferromagnets for spin-based technologies and applications. This article gives a broad perspective on antiferromagnetic spintronics. In particular, the manipulation and detection of antiferromagnetic states by spintronics effects, as well as spin transport and dynamics in antiferromagnetic materials will be discussed. We will also outline current challenges and future research directions in this emerging field.
Two-dimensional magnetism in the triangular antiferromagnet NiGa2S4
International Nuclear Information System (INIS)
Nambu, Yusuke
2013-01-01
At sufficiently low temperatures, electron spins in normal magnets generally order into some fashion, for instance, ferromagnetic and antiferromagnetic. Geometrical frustration and/or reduced dimensionality can suppress such conventional orders, and occasionally induce unknown states of matter. This is the case for the two-dimensional (2D) triangular antiferromagnet Ni(Ga 2 S 4 , in which S=1 nickel spins do not order, instead show an exotic magnetism. We found (1) a resonant critical slowing down toward T*=8.5 K followed by a viscous spin liquid behavior, and (2) a spin-size dependent ground state. To elucidate (1), spin dynamics ranging from 10 -13 to 10 0 seconds were quantitatively explored through the experimental techniques such as inelastic neutron scattering, backscattering, neutron spin echo, ac and nonlinear susceptibilities. The finding of (2) is evidenced by impurity effects. Integer spins substituted systems such as zinc and iron ions retain a quadratic temperature dependence of the magnetic specific heat as for the parent compound. However, substitutions of half-odd integer spins, cobalt and manganese ions, eventually induce a distinct behavior, indicating an importance of integer size of spins to stabilize the 2D magnetism realized in NiGa 2 S 4 . The article gives our experimental findings and as well as some relevant theoretical scenarios. (author)
Gradual pressure-induced change in the magnetic structure of the noncollinear antiferromagnet Mn3Ge
Sukhanov, A. S.; Singh, Sanjay; Caron, L.; Hansen, Th.; Hoser, A.; Kumar, V.; Borrmann, H.; Fitch, A.; Devi, P.; Manna, K.; Felser, C.; Inosov, D. S.
2018-06-01
By means of powder neutron diffraction we investigate changes in the magnetic structure of the coplanar noncollinear antiferromagnet Mn3Ge caused by an application of hydrostatic pressure up to 5 GPa. At ambient conditions the kagomé layers of Mn atoms in Mn3Ge order in a triangular 120∘ spin structure. Under high pressure the spins acquire a uniform out-of-plane canting, gradually transforming the magnetic texture to a noncoplanar configuration. With increasing pressure the canted structure fully transforms into the collinear ferromagnetic one. We observed that magnetic order is accompanied by a noticeable magnetoelastic effect, namely, spontaneous magnetostriction. The latter induces an in-plane magnetostrain of the hexagonal unit cell at ambient pressure and flips to an out-of-plane strain at high pressures in accordance with the change of the magnetic structure.
Czech Academy of Sciences Publication Activity Database
Jungwirth, Tomáš; Martí, Xavier; Wadley, P.; Wunderlich, Joerg
2016-01-01
Roč. 11, č. 3 (2016), 231-241 ISSN 1748-3387 R&D Projects: GA MŠk(CZ) LM2011026; GA ČR GB14-37427G EU Projects: European Commission(XE) 268066 - 0MSPIN Institutional support: RVO:68378271 Keywords : antiferromagnets * spintronics Subject RIV: BM - Solid Matter Physics ; Magnetism Impact factor: 38.986, year: 2016
Electric control of antiferromagnets
Fina, I.; Marti, X.
2016-01-01
In the past five years, most of the paradigmatic concepts employed in spintronics have been replicated substituting ferromagnets by antiferromagnets in critical parts of the devices. The numerous research efforts directed to manipulate and probe the magnetic moments in antiferromagnets have been gradually established a new and independent field known as antiferromagnetic spintronics. In this paper, we focus on the electrical control and detection of antiferromagnetic moments at a constant tem...
Magnetic study of a few antiferromagnets in very-strong pulsed fields (450 kOE)
International Nuclear Information System (INIS)
Krebs, J.
1968-01-01
In this thesis we describe a pulsed field device with which we obtain magnetization curves up to 450 kOE at all temperatures between 1. 6 and 300. We have studied the 'spin-flopping'(and therefore the anisotropy) in MnF 2 versus temperature, below the Neel point. We have also studied the antiferromagnets MnSO 4 . and MnSO 4 .H 2 O which have revealed saturation fields respectively of 250 kOE and 320 kOE. (author) [fr
International Nuclear Information System (INIS)
Machado, S.F.; Espirito Santo Univ., Vitoria; Tsallis, C.
1983-01-01
Within a mean field approximation, the influences of anisotropy (in the spin space) and external uniaxial stress on the Heisenberg antiferromagnet in the presence of magnetic field are discussed. The phase diagram evolution (as function of anisotropy and stress) which is obtained, enables a satisfactory overall interpretation of recent experiments on Mn(Br sub(1-x) Cl sub(x)) 2 .4H 2 O, K 2 [FeCl 5 (H 2 O)], CoCl 2 .6H 2 O and (C 2 H 5 NH 3 ) 2 CuCl 4 . (Author) [pt
Strong Coupling of Microwave Photons to Antiferromagnetic Fluctuations in an Organic Magnet
Mergenthaler, Matthias; Liu, Junjie; Le Roy, Jennifer J.; Ares, Natalia; Thompson, Amber L.; Bogani, Lapo; Luis, Fernando; Blundell, Stephen J.; Lancaster, Tom; Ardavan, Arzhang; Briggs, G. Andrew D.; Leek, Peter J.; Laird, Edward A.
2017-10-01
Coupling between a crystal of di(phenyl)-(2,4,6-trinitrophenyl)iminoazanium radicals and a superconducting microwave resonator is investigated in a circuit quantum electrodynamics (circuit QED) architecture. The crystal exhibits paramagnetic behavior above 4 K, with antiferromagnetic correlations appearing below this temperature, and we demonstrate strong coupling at base temperature. The magnetic resonance acquires a field angle dependence as the crystal is cooled down, indicating anisotropy of the exchange interactions. These results show that multispin modes in organic crystals are suitable for circuit QED, offering a platform for their coherent manipulation. They also utilize the circuit QED architecture as a way to probe spin correlations at low temperature.
International Nuclear Information System (INIS)
Ertaş Mehmet; Keskin Mustafa
2013-01-01
Using the mean-field theory and Glauber-type stochastic dynamics, we study the dynamic magnetic properties of the mixed spin (2, 5/2) Ising system for the antiferromagnetic/antiferromagnetic (AFM/AFM) interactions on the bilayer square lattice under a time varying (sinusoidal) magnetic field. The time dependence of average magnetizations and the thermal variation of the dynamic magnetizations are examined to calculate the dynamic phase diagrams. The dynamic phase diagrams are presented in the reduced temperature and magnetic field amplitude plane and the effects of interlayer coupling interaction on the critical behavior of the system are investigated. We also investigate the influence of the frequency and find that the system displays richer dynamic critical behavior for higher values of frequency than that of the lower values of it. We perform a comparison with the ferromagnetic/ferromagnetic (FM/FM) and AFM/FM interactions in order to see the effects of AFM/AFM interaction and observe that the system displays richer and more interesting dynamic critical behaviors for the AFM/AFM interaction than those for the FM/FM and AFM/FM interactions. (general)
Czech Academy of Sciences Publication Activity Database
Khmelevskyi, S.; Shick, Alexander; Mohn, P.
2011-01-01
Roč. 83, č. 22 (2011), "224419-1"-"224419-5" ISSN 1098-0121 R&D Projects: GA ČR(CZ) GAP204/10/0330; GA AV ČR IAA100100912 Institutional research plan: CEZ:AV0Z10100520 Keywords : magnetic anisotropy * antiferromagnetism Subject RIV: BM - Solid Matter Physics ; Magnetism Impact factor: 3.691, year: 2011
Modelling study of magnetic and concentration phase transition in ultrathin antiferromagnetic films
International Nuclear Information System (INIS)
Leonid, Afremov; Aleksandr, Petrov
2014-01-01
Using the method of the ''average spin'' a modelling study of magnetic and concentration phase transition in ultrathin antiferromagnetic of different crystalline structure has been carried out. It has been shown, that relative change of Neel temperature is subject to the power law with negative index which doesn't depend on the film's crystal kind. The calculation of the dependence of phase transition critical concentration in diluted magnetic material on the film thickness has been made out. The legitimacy of the use of the method developed for modelling of magnetic and concentration phase transition in different nanostructures is certified by accordance between the results of calculations and the experimental data
Tretiakov, Oleg; Barker, Joseph
Skyrmions are topologically protected entities in magnetic materials which have the potential to be used in spintronics for information storage and processing. However, skyrmions in ferromagnets have some intrinsic difficulties which must be overcome to use them for spintronic applications, such as the inability to move straight along current. We show that skyrmions can also be stabilized and manipulated in antiferromagnetic materials. An antiferromagnetic skyrmion is a compound topological object with a similar but of opposite sign spin texture on each sublattice, which e.g. results in a complete cancelation of the Magnus force. We find that the composite nature of antiferromagnetic skyrmions gives rise to different dynamical behavior, both due to an applied current and temperature effects. O.A.T. and J.B. acknowledge support by the Grants-in-Aid for Scientific Research (Nos. 25800184, 25247056, 25220910 and 15H01009) from the Ministry of Education, Culture, Sports, Science and Technology (MEXT) of Japan and SpinNet.
Wang, Wenqiang; Wang, Fenglong; Cao, Cuimei; Li, Pingping; Yao, Jinli; Jiang, Changjun
2018-04-01
CoZr/Ru/CoZr synthetic antiferromagnetic trilayers with strong antiferromagnetic interlayer coupling were fabricated by an oblique sputtering method that induced in-plane uniaxial magnetic anisotropy. A microstrip method using a vector network analyzer was applied to investigate the magnetic resonance modes of the trilayers, including the acoustic modes (AMs) and the optical modes (OMs). At zero magnetic field, the CoZr/Ru/CoZr trilayers showed OMs with resonance frequencies of up to 7.1 GHz. By increasing the applied external magnetic field, the magnetic resonance mode can be tuned to various OMs, mixed modes, and AMs. Additionally, the magnetic resonance mode showed an angular dependence between the magnetization and the microwave field, which showed similar switching of the magnetic modes with variation of the angle. Our results provide important information that will be helpful in the design of multifunctional microwave devices.
Akaki, M.; Tozawa, J.; Akahoshi, D.; Kuwahara, H.
2009-05-01
We have investigated the magnetic and dielectric properties of Ca2CoSi2O7 crystal. The dielectricity and magnetism of Ca2CoSi2O7 are strongly coupled below a canted antiferromagnetic transition temperature (TN). Magnetic fields induce electric polarization below TN. Interestingly, the magnetic-field-induced electric polarization is detected even without poling electric fields. Below TN, a canted antiferromagnetic-paramagnetic transition is induced by magnetic fields. The large magnetocapacitance is observed around TN. The origin of the large magnetocapacitance is due to the magnetic-field-induced the canted antiferromagnetic-paramagnetic transition.
Directory of Open Access Journals (Sweden)
Chong Wang
2013-12-01
Full Text Available We report on a spin-polarized inelastic neutron-scattering study of spin waves in the antiferromagnetically ordered state of BaFe_{2}As_{2}. Three distinct excitation components are identified, with spins fluctuating along the c axis, perpendicular to the ordering direction in the ab plane and parallel to the ordering direction. While the first two “transverse” components can be described by a linear spin-wave theory with magnetic anisotropy and interlayer coupling, the third “longitudinal” component is generically incompatible with the local-moment picture. It points toward a contribution of itinerant electrons to the magnetism that is already in the parent compound of this family of Fe-based superconductors.
Khmelevskyi, S; Mohn, P
2012-01-11
The investigation of the electronic structure and magnetism for the compound MnB(2) with crystal structure type AlB(2) has been revisited to resolve contradictions between various experimental and theoretical results present in the literature. We find that MnB(2) exhibits an interesting example of a Kübler's covalent magnetism (Williams et al 1981 J. Appl. Phys. 52 2069). The covalent magnetism also appears to be the source of some disagreement between the calculated values of the magnetic moments and those given by neutron diffraction experiments. We show that this shortcoming is due to the atomic sphere approximation applied in earlier calculations. The application of the disordered local moment approach and the calculation of the inter-atomic exchange interactions within the Liechtenstein formalism reveal strong local moment antiferromagnetism with a high Néel temperature predicted from Monte Carlo simulations. A fully relativistic band structure calculation and then the application of the torque method yields a strong in-plane anisotropy of the Mn magnetic moments. The agreement of these results with neutron diffraction studies rules out any possible weak itinerant electron magnetism scenarios as proposed earlier for MnB(2).
Magnetic anisotropy of the antiferromagnetic ring [Cr8F8Piv16].
van Slageren, Joris; Sessoli, Roberta; Gatteschi, Dante; Smith, Andrew A; Helliwell, Madeleine; Winpenny, Richard E P; Cornia, Andrea; Barra, Anne-Laure; Jansen, Aloysius G M; Rentschler, Eva; Timco, Grigore A
2002-01-04
A new tetragonal (P42(1)2) crystalline form of [Cr8F8Piv16] (HPiv = pivalic acid, trimethyl acetic acid) is reported. The ring-shaped molecules, which are aligned in a parallel fashion in the unit cell, form almost perfectly planar, regular octagons. The interaction between the CrIII ions is antiferromagnetic (J = 12 cm(-1)) which results in a S = 0 spin ground state. The low-lying spin excited states were investigated by cantilever torque magnetometry (CTM) and high-frequency EPR (HFEPR). The compound shows hard-axis anisotropy. The axial zero-field splitting (ZFS) parameters of the first two spin excited states (S = 1 and S = 2, respectively) are D1 = 1.59(3) cm(-1) or 1.63 cm(-1) (from CTM and HFEPR, respectively) and D2 = 0.37 cm(-1) (from HFEPR). The dipolar contributions to the ZFS of the S = 1 and S = 2 spin states were calculated with the point dipolar approximation. These contributions proved to be less than the combined single-ion contributions. Angular overlap model calculations that used parameters obtained from the electronic absorption spectrum, showed that the unique axis of the single-ion ZFS is at an angle of 19.3(1) degrees with respect to the ring axis. The excellent agreement between the experimental and the theoretical results show the validity of the used methods for the analysis of the magnetic anisotropy in antiferromagnetic CrIII rings.
Perspectives of antiferromagnetic spintronics
Energy Technology Data Exchange (ETDEWEB)
Jungfleisch, Matthias B.; Zhang, Wei; Hoffmann, Axel
2018-04-01
Antiferromagnets are promising for future spintronics applications owing to their interesting properties: They are magnetically ordered, but neighboring magnetic moments point in opposite directions which results in zero net magneti- zation. This means antiferromagnets produce no stray fields and are insensitive to external magnetic field perturbations. Furthermore, they show intrinsic high frequency dynamics, exhibit considerable spin-orbit and magneto-transport effects. Over the past decade, it has been realized that antiferromagnets have more to offer than just being utilized as passive components in exchange bias applications. This development resulted in a paradigm shift, which opens the pathway to novel concepts using antiferromagnets for spin-based technologies and applications. This article gives a broad per- spective on antiferromagnetic spintronics. In particular, the manipulation and detection of anitferromagnetic states by spintronics effects, as well as spin transport and dynamics in antiferromagnetic materials will be discussed. We will also outline current challenges and future research directions in this emerging field.
Magnetic ordering of quasi-1 D S=1/2 Heisenberg antiferromagnet Cu benzoate at sub-mK temperatures
International Nuclear Information System (INIS)
Karaki, Y.; Masutomi, R.; Kubota, M.; Ishimoto, H.; Asano, T.; Ajiro, Y.
2003-01-01
We have measured the AC susceptibility of quasi-1D S=1/2 Heisenberg antiferromagnet Cu benzoate at temperatures down to 0.2 mK. A sharp susceptibility peak is observed at 0.8 mK under an earth field. This fact indicates a 3D ordering of linear chains coupled by a weak magnetic interaction between chains
Spin frustration effects in an odd-member antiferromagnetic ring and the magnetic Mobius strip
International Nuclear Information System (INIS)
Cador, Olivier; Gatteschi, Dante; Sessoli, Roberta; Barra, Anne-Laure; Timco, Grigore A.; Winpenny, Richard E.P.
2005-01-01
The magnetic properties of the first odd-member antiferromagnetic ring comprising eight chromium(III) ions, S=32 spins, and one nickel(II) ion, S=1 spin, are investigated. The ring possesses an even number of unpaired electrons and a S=0 ground state but, due to competing AF interactions, the first excited spin states are close in energy. The spin frustrated ring is visualized by a Mobius strip. The 'knot' of the strip represents the region of the ring where the AF interactions are more frustrated. In the particular case of this bimetallic ring electron paramagnetic resonance (EPR) has unambiguously shown that the frustration is delocalized on the chromium chain, while the antiparallel alignment is more rigid at the nickel site
Spin frustration effects in an odd-member antiferromagnetic ring and the magnetic Mobius strip
Energy Technology Data Exchange (ETDEWEB)
Cador, Olivier [Laboratory of Molecular Magnetism, Department of Chemistry and UdR INSTM, Universita degli Studi di Firenze, Via Lastruccia n. 3, 50019 Sesto Fiorentino (Italy); Gatteschi, Dante [Laboratory of Molecular Magnetism, Department of Chemistry and UdR INSTM, Universita degli Studi di Firenze, Via Lastruccia n. 3, 50019 Sesto Fiorentino (Italy); Sessoli, Roberta [Laboratory of Molecular Magnetism, Department of Chemistry and UdR INSTM, Universita degli Studi di Firenze, Via Lastruccia n. 3, 50019 Sesto Fiorentino (Italy)]. E-mail: roberta.sessoli@unifi.it; Barra, Anne-Laure [Laboratoire des Champs Magnetiques Intenses-CNRS, F-38042 Grenoble Cede 9 (France); Timco, Grigore A. [Department of Chemistry, University of Manchester, Oxford Road, Manchester M13 9PL (United Kingdom); Winpenny, Richard E.P. [Department of Chemistry, University of Manchester, Oxford Road, Manchester M13 9PL (United Kingdom)
2005-04-15
The magnetic properties of the first odd-member antiferromagnetic ring comprising eight chromium(III) ions, S=32 spins, and one nickel(II) ion, S=1 spin, are investigated. The ring possesses an even number of unpaired electrons and a S=0 ground state but, due to competing AF interactions, the first excited spin states are close in energy. The spin frustrated ring is visualized by a Mobius strip. The 'knot' of the strip represents the region of the ring where the AF interactions are more frustrated. In the particular case of this bimetallic ring electron paramagnetic resonance (EPR) has unambiguously shown that the frustration is delocalized on the chromium chain, while the antiparallel alignment is more rigid at the nickel site.
Kuiper, Pieter; Searle, Barry G.; Rudolf, Petra; Tjeng, L.H.; Chen, C.T.
1993-01-01
We report strong magnetic linear dichroism at the Fe L2,3 edge of the antiferromagnet Fe2O3 (hematite). The relative difference in absorption for light polarized parallel and perpendicular to the magnetic moment is as high as 40% at the Fe L2 edge. The spectra are in excellent agreement with
International Nuclear Information System (INIS)
Erdinc, Ahmet; Canko, Osman; Keskin, Mustafa
2006-01-01
We have studied the antiferromagnetic Blume-Emery-Griffiths model with the repulsive biquadratic coupling in an external magnetic field using the lowest approximation of the cluster variation method which is identical to the mean-field approximation. First, we have investigated the thermal variations of the sublattice magnetizations and obtained four different main topological types. Then, we have calculated the phase diagrams and five main different phase diagram topologies are found. Finally, the discussion and comparison of the phase diagrams are made
Energy Technology Data Exchange (ETDEWEB)
Erdinc, Ahmet [Department of Physics, Erciyes University, 38039 Kayseri (Turkey); Canko, Osman [Department of Physics, Erciyes University, 38039 Kayseri (Turkey); Keskin, Mustafa [Department of Physics, Erciyes University, 38039 Kayseri (Turkey)]. E-mail: keskin@erciyes.edu.tr
2006-06-15
We have studied the antiferromagnetic Blume-Emery-Griffiths model with the repulsive biquadratic coupling in an external magnetic field using the lowest approximation of the cluster variation method which is identical to the mean-field approximation. First, we have investigated the thermal variations of the sublattice magnetizations and obtained four different main topological types. Then, we have calculated the phase diagrams and five main different phase diagram topologies are found. Finally, the discussion and comparison of the phase diagrams are made.
Surface-spin magnetism of antiferromagnetic NiO in nanoparticle and bulk morphology
International Nuclear Information System (INIS)
Jagodic, M; Jaglicic, Z; Jelen, A; Dolinsek, J; Lee, Jin Bae; Kim, Hae Jin; Kim, Young-Min
2009-01-01
The surface-spin magnetism of the antiferromagnetic (AFM) material NiO in nanoparticle and bulk morphology was investigated by magnetic measurements (temperature-dependent zero-field-cooled (zfc) and field-cooled (fc) dc susceptibility, ac susceptibility and zfc and fc hysteresis loops). We addressed the question of whether the multisublattice ordering of the uncompensated surface spins and the exchange bias (EB) effect are only present in the nanoparticles, originating from their high surface-to-volume ratio or if these surface phenomena are generally present in the AFM materials regardless of their bulky or nanoparticle morphology, but the effect is just too small to be detected experimentally in the bulk due to a very small surface magnetization. Performing experiments on the NiO nanoparticles of different sizes and bulk NiO grains, we show that coercivity enhancement and hysteresis loop shift in the fc experiments, considered to be the key experimental manifestations of multisublattice ordering and the EB effect, are true nanoscale phenomena only present in the nanoparticles and absent in the bulk.
International Nuclear Information System (INIS)
Lee, J. Y.; Guan, X. W.; Batchelor, M. T.; Lee, C.
2009-01-01
We investigate magnetism and quantum phase transitions in a one-dimensional system of integrable spin-1 bosons with strongly repulsive density-density interaction and antiferromagnetic spin-exchange interaction via the thermodynamic Bethe ansatz method. At zero temperature, the system exhibits three quantum phases: (i) a singlet phase of boson pairs when the external magnetic field H is less than the lower critical field H c1 ; (ii) a ferromagnetic phase of atoms in the hyperfine state |F=1, m F =1> when the external magnetic field exceeds the upper critical field H c2 ; and (iii) a mixed phase of singlet pairs and unpaired atoms in the intermediate region H c1 c2 . At finite temperatures, the spin fluctuations affect the thermodynamics of the model through coupling the spin bound states to the dressed energy for the unpaired m F =1 bosons. However, such spin dynamics is suppressed by a sufficiently strong external field at low temperatures. Thus the singlet pairs and unpaired bosons may form a two-component Luttinger liquid in the strong coupling regime.
Directory of Open Access Journals (Sweden)
Youhei Yamaji
2014-05-01
Full Text Available Topological insulators, in contrast to ordinary semiconductors, accompany protected metallic surfaces described by Dirac-type fermions. Here, we theoretically show that another emergent two-dimensional metal embedded in the bulk insulator is realized at a magnetic domain wall. The domain wall has long been studied as an ingredient of both old-fashioned and leading-edge spintronics. The domain wall here, as an interface of seemingly trivial antiferromagnetic insulators, emergently realizes a functional interface preserved by zero modes with robust two-dimensional Fermi surfaces, where pyrochlore iridium oxides proposed to host the condensed-matter realization of Weyl fermions offer such examples at low temperatures. The existence of in-gap states that are pinned at domain walls, theoretically resembling spin or charge solitons in polyacetylene, and protected as the edges of hidden one-dimensional weak Chern insulators characterized by a zero-dimensional class-A topological invariant, solves experimental puzzles observed in R_{2}Ir_{2}O_{7} with rare-earth elements R. The domain wall realizes a novel quantum confinement of electrons and embosses a net uniform magnetization that enables magnetic control of electronic interface transports beyond the semiconductor paradigm.
Spintronics of antiferromagnetic systems
International Nuclear Information System (INIS)
Gomonaj, E.V.; Loktev, V.M.
2014-01-01
Spintronics of antiferromagnetics is a new field that has developed in a fascinating research topic in physics of magnetism. Antiferromagnetics, like ferromagnetic materials experience the influence of spin-polarized current, even though they show no macroscopic magnetization. The mechanism of this phenomenon is related to spin-dependent interaction between free and localized electrons-sd-exchange. Due to the peculiarities of antiferromagnetic materials (complicated magnetic structure, essential role of the exchange interactions, lack of macroscopic magnetization) spintronics of antiferromagnets appeals to new theoretical and experimental approaches. The purpose of this review is to systemize and summarize the recent progress in this field. We start with a short introduction into the structure and dynamics of antiferromagnets and proceed with discussion of different microscopic and phenomenological theories for description of current-induced phenomena in ferro-/antiferromagnetic heterostructures. We also consider the problems of the reverse influence of antiferromagnetic ordering on current, and effectiveness of the fully antiferromagnetic spin valve. In addition, we shortly review and interpret the available experimental results.
Wang, Zhe; Lorenz, T.; Gorbunov, D. I.; Cong, P. T.; Kohama, Y.; Niesen, S.; Breunig, O.; Engelmayer, J.; Herman, A.; Wu, Jianda; Kindo, K.; Wosnitza, J.; Zherlitsyn, S.; Loidl, A.
2018-05-01
We report on magnetization, sound-velocity, and magnetocaloric-effect measurements of the Ising-like spin-1 /2 antiferromagnetic chain system BaCo2V2O8 as a function of temperature down to 1.3 K and an applied transverse magnetic field up to 60 T. While across the Néel temperature of TN˜5 K anomalies in magnetization and sound velocity confirm the antiferromagnetic ordering transition, at the lowest temperature the field-dependent measurements reveal a sharp softening of sound velocity v (B ) and a clear minimum of temperature T (B ) at B⊥c,3 D=21.4 T , indicating the suppression of the antiferromagnetic order. At higher fields, the T (B ) curve shows a broad minimum at B⊥c=40 T , accompanied by a broad minimum in the sound velocity and a saturationlike magnetization. These features signal a quantum phase transition, which is further characterized by the divergent behavior of the Grüneisen parameter ΓB∝(B -B⊥c)-1. By contrast, around the critical field, the Grüneisen parameter converges as temperature decreases, pointing to a quantum critical point of the one-dimensional transverse-field Ising model.
[mu]SR magnetic response in frustrated antiferromagnets of type RMn[sub 2] (R = rare earth)
Energy Technology Data Exchange (ETDEWEB)
Weber, M. (Physics Dept., TU Munich, Garching (Germany)); Asch, L. (Physics Dept., TU Munich, Garching (Germany)); Kratzer, A. (Physics Dept., TU Munich, Garching (Germany)); Kalvius, G.M. (Physics Dept., TU Munich, Garching (Germany)); Muench, K.H. (Physics Dept., TU Munich, Garching (Germany)); Ballou, R. (Lab. Louis Neel, CNRS, 38 Grenoble (France)); Deportes, J. (Lab. Louis Neel, CNRS, 38 Grenoble (France)); Waeppling, R. (Dept. of Physics, Univ. of Uppsala (Sweden)); Litterst, F.J. (Inst. for Metal Physics, TU Braunschweig (Germany)); Klauss, H.H. (Inst. for Metal Physics, TU Braunschweig (Germany)); Niedermayer, C. (Faculty for Physics, Univ. Konstanz (Germany)); Chappert, J. (CEA/DRFMC, CEN Grenoble, 38 (France))
1994-07-01
Zero, longitudinal and transverse field [mu]SR was carried out in the antiferromagnets YMn[sub 2], Y[sub 0.95] Tb[sub 0.15] Mn[sub 2], Y[sub 0.9]Tb[sub 0.1]Mn[sub 2], Y[sub 0.99] Sc[sub 0.01] Mn[sub 2], Y[sub 0.98]Sc[sub 0.02]Mn[sub 2] and TbMn[sub 2]. The dynamics of Mn magnetic moments above T[sub N] is typical for an itinerant antiferromagnet. Within a certain temperature range above T[sub N] part of the material enters a randomly ordered (spin glass like) magnetic state as an out-come of frustration. At temperatures above [approx] 150 K the muon spin relaxation rate indicates that the muon has become mobile. (orig.)
Spin-flip transition and Faraday effect in antiferromagnet KMnF3 in megagauss magnetic field
International Nuclear Information System (INIS)
Mukhin, A.A.; Plis, V.I.; Popov, A.I.; Zvezdin, A.K.; Platonov, V.; Tatsenko, O.M.
1998-01-01
Faraday effect in the antiferromagnet KMnF 3 has been investigated in pulse explosive fields up to 500 T at T=78 K. The laser wavelength 0.63 μm was used in the experiment. The magnetic field dependence of Faraday rotation in this antiferromagnet shows a unique feature of a lack of saturation effect in the fields up to 500 T whereas critical field of spin-flip transition is about 120 T. The theoretical analysis of microscopic nature of Faraday rotation, including the diamagnetic, magneto-dipole and paramagnetic mechanisms has been performed. The strong competition of these mechanisms is important to explain the extremely small value of the effect and its unusual magnetic field dependence
Magnetic properties of CsCrCl/sub 3/, an antiferromagnetic chain compound with single-ion anisotropy
Energy Technology Data Exchange (ETDEWEB)
Day, P; Gregson, A K; Leech, D H [Oxford Univ. (UK). Inorganic Chemistry Lab.; Hutchings, M T [UKAEA Atomic Energy Research Establishment, Harwell. Materials Physics Div.; Rainford, B D [Imperial Coll. of Science and Technology, London (UK). Dept. of Physics
1979-01-01
The magnetic structure and excitations of the linear chain hexagonal perovskite salt CsCrCl/sub 3/ have been studied by susceptibility, powder and single crystal neutron diffraction, and coherent inelastic neutron scattering. Below the Neel temperature, Tsub(N) = 16 K, the spins lie in the basal plane with antiferromagnetic ordering along the c-axis chains. At 4.5 K there is strong dispersion of the spin-wave energy along c but no measurable dispersion perpendicular to c.
Directory of Open Access Journals (Sweden)
Qiang Hao
2016-02-01
Full Text Available We investigate the magnetic stability and endurance of MgO-based magnetic tunnel junctions (MTJs with an exchange-biased synthetic antiferromagnetic (SAF pinned layer. When a uniaxially cycling switching field is applied along the easy axis of the free magnetic layer, the magnetoresistance varies only by 1.7% logarithmically with the number of cycles, while no such change appears in the case of a rotating field. This observation is consistent with the effect of the formation and motion of domain walls in the free layer, which create significant stray fields within the pinned hard layer. Unlike in previous studies, the decay we observed only occurs during the first few starting cycles (<20, at which point there is no further variance in all performance parameters up to 107 cycles. Exchange-biased SAF structure is ideally suited for solid-state magnetic sensors and magnetic memory devices.
Effect of Dzyaloshinskii-Moriya on Magnetic orders of J_1-J_2 Antiferromagnetic Heisenberg model
Directory of Open Access Journals (Sweden)
Fariba Masoudi
2017-11-01
Full Text Available Motivated by recent experiments that detects Dzyaloshinskii-Moriya (DM interaction in , we study the effects of DM interaction on magnetic orders of J1-J2 antiferromagnetic Heisenberg model. First, we find the classical phase diagram of the model using Luttinger-Tisza approximation. In this approximation, the classical phase diagram has two phases. For , the model has canted Neel and DM interaction cants the spins of one on the subluttices. The ground state of model is classically degenerate for , including infinit numbers of vorticity vectors that are able to minimize the model. This phase is important because of the probability of the existence of quantum spin liquid in this region. To investigate the effect of quantum fluctuation on the stability of the classical phase diagram, linear spin wave theory of Holstein-Primakoff is used. The results show that in the classical degeneracy regime, the quantum fluctuations for cause spiral order in this region. The ground state of model remains disorder for, and this region is a good place for finding quantum spin liquid
Reentrant behavior in the nearest-neighbor Ising antiferromagnet in a magnetic field
Neto, Minos A.; de Sousa, J. Ricardo
2004-12-01
Motived by the H-T phase diagram in the bcc Ising antiferromagnetic with nearest-neighbor interactions obtained by Monte Carlo simulation [Landau, Phys. Rev. B 16, 4164 (1977)] that shows a reentrant behavior at low temperature, with two critical temperatures in magnetic field about 2% greater than the critical value Hc=8J , we apply the effective field renormalization group (EFRG) approach in this model on three-dimensional lattices (simple cubic-sc and body centered cubic-bcc). We find that the critical curve TN(H) exhibits a maximum point around of H≃Hc only in the bcc lattice case. We also discuss the critical behavior by the effective field theory in clusters with one (EFT-1) and two (EFT-2) spins, and a reentrant behavior is observed for the sc and bcc lattices. We have compared our results of EFRG in the bcc lattice with Monte Carlo and series expansion, and we observe a good accordance between the methods.
Bernot, K.; Luzon, J.; Caneschi, A.; Gatteschi, D.; Sessoli, R.; Bogani, L.; Vindigni, A.; Rettori, A.; Pini, M. G.
2009-04-01
We investigate theoretically and experimentally the static magnetic properties of single crystals of the molecular-based single-chain magnet of formula [Dy(hfac)3NIT(C6H4OPh)]∞ comprising alternating Dy3+ and organic radicals. The magnetic molar susceptibility χM displays a strong angular variation for sample rotations around two directions perpendicular to the chain axis. A peculiar inversion between maxima and minima in the angular dependence of χM occurs on increasing temperature. Using information regarding the monomeric building block as well as an ab initio estimation of the magnetic anisotropy of the Dy3+ ion, this “anisotropy-inversion” phenomenon can be assigned to weak one-dimensional ferromagnetism along the chain axis. This indicates that antiferromagnetic next-nearest-neighbor interactions between Dy3+ ions dominate, despite the large Dy-Dy separation, over the nearest-neighbor interactions between the radicals and the Dy3+ ions. Measurements of the field dependence of the magnetization, both along and perpendicularly to the chain, and of the angular dependence of χM in a strong magnetic field confirm such an interpretation. Transfer-matrix simulations of the experimental measurements are performed using a classical one-dimensional spin model with antiferromagnetic Heisenberg exchange interaction and noncollinear uniaxial single-ion anisotropies favoring a canted antiferromagnetic spin arrangement, with a net magnetic moment along the chain axis. The fine agreement obtained with experimental data provides estimates of the Hamiltonian parameters, essential for further study of the dynamics of rare-earth-based molecular chains.
Magnetic order, magnetic correlations, and spin dynamics in the pyrochlore antiferromagnet Er2Ti2O7
Dalmas de Réotier, P.; Yaouanc, A.; Chapuis, Y.; Curnoe, S. H.; Grenier, B.; Ressouche, E.; Marin, C.; Lago, J.; Baines, C.; Giblin, S. R.
2012-09-01
Er2Ti2O7 is believed to be a realization of an XY antiferromagnet on a frustrated lattice of corner-sharing regular tetrahedra. It is presented as an example of the order-by-disorder mechanism in which fluctuations lift the degeneracy of the ground state, leading to an ordered state. Here we report detailed measurements of the low-temperature magnetic properties of Er2Ti2O7, which displays a second-order phase transition at TN≃1.2 K with coexisting short- and long-range orders. Magnetic susceptibility studies show that there is no spin-glass-like irreversible effect. Heat capacity measurements reveal that the paramagnetic critical exponent is typical of a 3-dimensional XY magnet while the low-temperature specific heat sets an upper limit on the possible spin-gap value and provides an estimate for the spin-wave velocity. Muon spin relaxation measurements show the presence of spin dynamics in the nanosecond time scale down to 21 mK. This time range is intermediate between the shorter time characterizing the spin dynamics in Tb2Sn2O7, which also displays long- and short-range magnetic order, and the time scale typical of conventional magnets. Hence the ground state is characterized by exotic spin dynamics. We determine the parameters of a symmetry-dictated Hamiltonian restricted to the spins in a tetrahedron, by fitting the paramagnetic diffuse neutron scattering intensity for two reciprocal lattice planes. These data are recorded in a temperature region where the assumption that the correlations are limited to nearest neighbors is fair.
Induced magnetic structure in exchange-coupled ferro-/antiferromagnet thin films
Morales, Rafael
2007-03-01
The most prominent feature observed in exchange-coupled ferromagnetic/ antiferromagnetic (FM/AF) bilayers is the so-called exchange bias field (HEB), i.e. the shift of the hysteresis loop along the magnetic field axis. However the exchange bias phenomenon can induce other interesting effects on the FM. In this talk we show two methods to establish a bi-domain state in the FM, due to the coexistence of domains with opposite sign of HEB [1-3]. Magneto-optical, polarized neutron and soft X-ray measurements show that this lateral structure becomes more complex for low magnetocrystalline anisotropy materials where a spin depth profile is created in the FM due to the exchange coupling with the AF [4-6]. The internal magnetic structure in the AF and its role on exchange bias has also been investigated using FM/AF/FM trilayers. These studies demonstrate that the bulk spin configuration in the AF plays a crucial role in the pinning of uncompensated spins at the interface thus determining the HEB . Supported by the US-DOE, European Marie-Curie-OIF and the Alfred P. Sloan Foundation. [1] O. Petracic et al. Appl. Phys. Lett. 87, 222509 (2005) [2] I. V. Roshchin et al. Europhys. Lett. 71, 297 (2005) [3] J. Olamit et al. Phys. Rev. B 72, 012408 (2005) [4] R. Morales et al. Appl. Phys. Lett. 89, 072504 (2006) [5] S. Roy et al. Phys. Rev. Lett. 95, 047201 (2005) [6] Z-P. Li et al. Phys. Rev. Lett. 96, 217205 (2006)
One- and Two- Magnon Excitations in a One-Dimensional Antiferromagnet in a Magnetic Field
DEFF Research Database (Denmark)
Heilmann, I.U.; Kjems, Jørgen; Endoh, Y.
1981-01-01
We have carried out a comprehensive experimental and theoretical study of the inelastic scattering in the one-dimensional near-Heisenberg antiferromagnet (CD3)4NMnCl3 (TMMC) at low temperatures, 0.3...
Magnetic behavior of the diluted antiferromagnet Mn0.39Zn0.61F2 at strong fields
International Nuclear Information System (INIS)
Rosales-Rivera, A.; Ferreira, J.M.; Montenegro, F.C.; Ramos, C.A.
2001-01-01
The magnetic phase boundaries of the random-field Ising model (RFIM) system Mn 0.39 Zn 0.61 F 2 are determined using magnetization measurements, under finite DC applied fields (H). At low fields (H<12 kOe), our results support a critical phase boundary, separating an ordered antiferromagnetic (AF) phase from the paramagnetic (P) one. For intermediate fields (12< H<18 kOe), the AF ordering coexists with a spin-flop (SF) clustering. For higher H, a spin-flop phase dominates the upper part of the (H,T) phase diagram
Field-induced magnetic instability and quantum criticality in the antiferromagnet CeCu2Ge2.
Liu, Yi; Xie, Donghua; Wang, Xiaoying; Zhu, Kangwei; Yang, Ruilong
2016-01-13
The magnetic quantum criticality in strongly correlated electron systems has been considered to be closely related with the occurrence of unconventional superconductivity. Control parameters such as magnetic field, pressure or chemical doping are frequently used to externally tune the quantum phase transition for a deeper understanding. Here we report the research of a field-induced quantum phase transition using conventional bulk physical property measurements in the archetypal antiferromagnet CeCu2Ge2, which becomes superconductive under a pressure of about 10 GPa with Tc ~ 0.64 K. We offer strong evidence that short-range dynamic correlations start appearing above a magnetic field of about 5 T. Our demonstrations of the magnetic instability and the field-induced quantum phase transition are crucial for the quantum criticality, which may open a new route in experimental investigations of the quantum phase transition in heavy-fermion systems.
Energy Technology Data Exchange (ETDEWEB)
Blundell, S.J.; Pratt, F.L.; Lancaster, T.; Marshall, I.M.; Steer, C.A.; Hayes, W.; Sugano, T.; Letard, J.-F.; Caneschi, A.; Gatteschi, D.; Heath, S.L
2003-02-01
We present the results of recent {mu}SR experiments on a variety of novel organic and molecular magnetic systems. Muons are sensitive to local static fields and magnetic fluctuations, but can probe much more than just the onset of long-range magnetic order. We review our work on nitronyl nitroxide organic ferromagnets and antiferromagnets. We describe a muon study of the spin-crossover phenomenon which has been studied in Fe(PM-PEA){sub 2}(NCS){sub 2}, and which shows Gaussian and root-exponential muon relaxation in the high-spin and low-spin phases, respectively. Experiments on a disc-shaped molecular complex containing Fe{sub 19} (with spin ((31)/(2))) reveal the effects of quantum tunneling of magnetization and allow an estimate of the quantum tunneling rate.
International Nuclear Information System (INIS)
Blundell, S.J.; Pratt, F.L.; Lancaster, T.; Marshall, I.M.; Steer, C.A.; Hayes, W.; Sugano, T.; Letard, J.-F.; Caneschi, A.; Gatteschi, D.; Heath, S.L.
2003-01-01
We present the results of recent μSR experiments on a variety of novel organic and molecular magnetic systems. Muons are sensitive to local static fields and magnetic fluctuations, but can probe much more than just the onset of long-range magnetic order. We review our work on nitronyl nitroxide organic ferromagnets and antiferromagnets. We describe a muon study of the spin-crossover phenomenon which has been studied in Fe(PM-PEA) 2 (NCS) 2 , and which shows Gaussian and root-exponential muon relaxation in the high-spin and low-spin phases, respectively. Experiments on a disc-shaped molecular complex containing Fe 19 (with spin ((31)/(2))) reveal the effects of quantum tunneling of magnetization and allow an estimate of the quantum tunneling rate
Magnetization plateaus in the spin-1/2 antiferromagnetic Heisenberg model on a kagome-strip chain
Morita, Katsuhiro; Sugimoto, Takanori; Sota, Shigetoshi; Tohyama, Takami
2018-01-01
The spin-1/2 Heisenberg model on a kagome lattice is a typical frustrated quantum spin system. The basic structure of a kagome lattice is also present in the kagome-strip lattice in one dimension, where a similar type of frustration is expected. We thus study the magnetization plateaus of the spin-1/2 Heisenberg model on a kagome-strip chain with three-independent antiferromagnetic exchange interactions using the density-matrix renormalization-group method. In a certain range of exchange parameters, we find twelve kinds of magnetization plateaus, nine of which have magnetic structures breaking translational and/or reflection symmetry spontaneously. The structures are classified by an array of five-site unit cells with specific bond-spin correlations. In a case with a nontrivial plateau, namely a 3/10 plateau, we find long-period magnetic structure with a period of four unit cells.
Magnetic Field Enhancement of Heat Transport in the 2D Heisenberg Antiferromagnet K_2V_3O_8
Sales, B. C.; Lumsden, M. D.; Nagler, S. E.; Mandrus, D.; Jin, R.
2002-03-01
The thermal conductivity and heat capacity of single crystals of the spin 1/2 quasi-2D Heisenberg antiferromagnet K_2V_3O8 have been measured from 1.9 to 300 K in magnetic fields from 0 to 8T. The data are consistent with resonant scattering of phonons by magnons near the zone boundary and heat transport by long wavelength magnons. The magnon heat transport only occurs after the small anisotropic gap at k=0 is closed by the application of a magnetic field. The low temperature thermal conductivity increases linearly with magnetic field after the gap has been closed. Oak Ridge National Laboratory is managed by UT-Battelle LLC for the U.S. Department of Energy under Contract No. DE-AC05-00R22725.
Magnetic behaviour of the honeycomb antiferromagnet BaNi{sub 2}V{sub 2}O{sub 8}
Energy Technology Data Exchange (ETDEWEB)
Klyushina, Ekaterina; Lake, Bella [Helmholtz-Zentrum Berlin fuer Materialien und Energie, Berlin (Germany); Institut fuer Festkoerperphysik, Technische Universitaet Berlin, Berlin (Germany); Islam, Nazmul; Klemke, Bastian [Helmholtz-Zentrum Berlin fuer Materialien und Energie, Berlin (Germany); Schneidewind, Astrid; Park, Jitae [Heinz Maier-Leibnitz Zentrum, TU Muenchen, Garching (Germany); Mansson, Martin [Paul Scherrer Institute (Switzerland)
2016-07-01
Here we present our recent investigations of a spin-1 honeycomb antiferromagnetic BaNi{sub 2}V{sub 2}O{sub 8} which is a highly 2D antiferromagnet with XY anisotropy making this compound a potential candidate for the Berezinsky-Kosterliz-Thouless topological phase transition. Single crystal inelastic neutron scattering measurements in the honeycomb plane at 4 K reveal that the magnetic excitations extend from 0.3-26 meV and consist of two anisotropy-split gapped modes with gaps of 0.3 meV and 3.3 meV arising from the anisotropy within the a-b plane and XY anisotropy respectively. The excitations agree well with simulations based on linear spin - wave theory and are completely dispersionless in the out-of-plane direction suggesting negligible interplane coupling in spite of the long range magnetic order below T{sub N} = 48 K. A detailed investigation of the order parameter and correlation length are presented and compared to various theories.
DEFF Research Database (Denmark)
Zaharko, O.; Cervellino, A.; Tsurkan, V.
2010-01-01
Using neutron powder diffraction and Monte Carlo simulations we show that a spin-liquid regime emerges at all compositions in the diamond-lattice antiferromagnets Co(Al1−xCox)2O4. This spin-liquid regime induced by frustration due to the second-neighbor exchange coupling J2 is gradually superseded...... by antiferromagnetic collinear long-range order (k=0) at low temperatures. Upon substitution of Al3+ by Co3+ in the octahedral B site the temperature range occupied by the spin-liquid regime narrows and TN increases. To explain the experimental observations we considered magnetic anisotropy D or third......-neighbor exchange coupling J3 as degeneracy-breaking perturbations. We conclude that Co(Al1−xCox)2O4 is below the theoretical critical point J2/J1=1/8, and that magnetic anisotropy assists in selecting a collinear long-range ordered ground state, which becomes more stable with increasing x due to a higher...
Wu, Hashen; Kawakami, Daisuke; Sasaki, Mari; Xie, Jimin; Takaishi, Shinya; Kajiwara, Takashi; Miyasaka, Hitoshi; Yamashita, Masahiro; Matsuzaki, Hiroyuki; Okamoto, Hiroshi
2007-09-03
The disordered patterns of R- and rac-1,2-diaminopropane (pn) in quasi-one-dimensional bromo-bridged Ni(III) complexes, [NiIII(pn)2Br]Br2, have been investigated by single-crystal X-ray structure determination and scanning tunneling microscopy (STM). X-ray structure determination shows that the methyl moieties are disordered on the right- and left-hand sides with half occupancies in both compounds, while the carbon atoms of the ethylene moieties of pn ligands are disordered in [Ni(rac-pn)2Br]Br2 and not disordered in [Ni(R-pn)2Br]Br2. In the STM images of both compounds, the bright spots are not straight but fluctuated with the similar patterns. We have concluded that tunnel current from the STM tip to metal ions are detected via methyl groups of pn ligands.
International Nuclear Information System (INIS)
Terai, Tomoyuki; Yasui, Motoyoshi; Yamamoto, Masataka; Kakeshita, Tomoyuki
2009-01-01
We have investigated the rearrangement of crystallographic domains (martensite variants) in Ni 2 MnGa ferromagnetic shape memory alloy and CoO antiferromagnetic oxide by applying magnetic field up to 8.0 MA/m. From the result of optical microscope observation of Ni 2 MnGa single crystal, when a magnetic field is applied along [001] p (p represents a parent phase), the rearrangement of crystallographic domains occurs and the single domain state is obtained below T Ms = 202 K. The same rearrangement occurs but partially when a magnetic field is applied along [110] p . On the other hand, when a magnetic field is applied along [111] p , the rearrangement does not occur. In case of the CoO single crystal, when a magnetic field is applied along [001] p below T Ms = 293 K, the rearrangement occurs at 170 K ≤ T ≤ 293 K, but does not occur at T p and [111] p , the rearrangement does not occur below T Ms . In order to explain the rearrangement in the alloy and the oxide, we have evaluated the magnetic shear stress, τ mag , which is derived from the difference in magnetic energy among crystallographic domains and have compared it with the shear stress required for the twinning plane movement, τ req . As a result, we have found that the rearrangement occurs when the value of τ mag is larger than or equal to the value of τ req for the present alloy and oxide.
Effects of geometry in itinerant electron magnets
Energy Technology Data Exchange (ETDEWEB)
Nakamura, H [Graduate School of Material Science, University of Hyogo, Kamigori, Ako-gun, Hyogo 678-1297 (Japan); Muro, Y [Graduate School of Material Science, University of Hyogo, Kamigori, Ako-gun, Hyogo 678-1297 (Japan); Kohara, T [Graduate School of Material Science, University of Hyogo, Kamigori, Ako-gun, Hyogo 678-1297 (Japan); Shiga, M [Department of Materials Science and Engineering, Kyoto University, Kyoto 606-8501 (Japan)
2007-04-11
The magnetism of quasi-one-dimensional itinerant electron magnets RMn{sub 4}Al{sub 8} is compared with that of the typical frustrated itinerant electron magnet YMn{sub 2}. The possible formation and observation of the spin pseudogap are discussed in connection with the spin-liquid state in strongly correlated itinerant electron systems.
Morinari, Takao
2018-06-01
The central issue in high-temperature cuprate superconductors is the pseudogap state appearing below the pseudogap temperature T*, which is well above the superconducting transition temperature. In this study, we theoretically investigate the rapid increase of the magnetic anisotropy below the pseudogap temperature detected by the recent torque-magnetometry measurements on YBa2Cu3Oy [Y. Sato et al., 10.1038/nphys4205" xlink:type="simple">Nat. Phys. 13, 1074 (2017)]. Applying the spin Green's function formalism including the Dzyaloshinskii-Moriya interaction arising from the buckling of the CuO2 plane, we obtain results that are in good agreement with the experiment and find a scaling relationship. Our analysis suggests that the characteristic temperature associated with the magnetic anisotropy, which coincides with T*, is not a phase transition temperature but a crossover temperature associated with the short-range antiferromagnetic order.
Quasi-1D s=1/2 antiferromagnet Cs2CuCl4 in a magnetic field
DEFF Research Database (Denmark)
Coldea, R.; Tennant, D.A.; Cowley, R.A.
1997-01-01
than the field (similar or equal to 8 T) required to fully align the spins, are observed to decouple the chains, and the system enters a disordered intermediate-field phase (IFP). The IFP excitations are in agreement with the predictions of Muller et al. for the 1D S = 1/2 HAF, and Talstra and Haldane......Magnetic excitations of the quasi-1D S = 1/2 Heisenberg antiferromagnet (HAF) Cs2CuCl4 have beer measured as a function of magnetic field using neutron scattering. For T Fields greater than B-c = 1.66 T, but less...... for the related l/r(2) chain (the Haldane-Shastry model). This behavior is inconsistent with linear spin-wave theory....
Magnetic imaging of antiferromagnetic and superconducting phases in R bxF e2 -yS e2 crystals
Hazi, J.; Mousavi, T.; Dudin, P.; van der Laan, G.; Maccherozzi, F.; Krzton-Maziopa, A.; Pomjakushina, E.; Conder, K.; Speller, S. C.
2018-02-01
High-temperature superconducting (HTS) cuprate materials, with the ability to carry large electrical currents with no resistance at easily reachable temperatures, have stimulated enormous scientific and industrial interest since their discovery in the 1980's. However, technological applications of these promising compounds have been limited by their chemical and microstructural complexity and the challenging processing strategies required for the exploitation of their extraordinary properties. The lack of theoretical understanding of the mechanism for superconductivity in these HTS materials has also hindered the search for new superconducting systems with enhanced performance. The unexpected discovery in 2008 of HTS iron-based compounds has provided an entirely new family of materials for studying the crucial interplay between superconductivity and magnetism in unconventional superconductors. Alkali-metal-doped iron selenide (AxF e2 -yS e2 , A =alkali metal ) compounds are of particular interest owing to the coexistence of superconductivity at relatively high temperatures with antiferromagnetism. Intrinsic phase separation on the mesoscopic scale is also known to occur in what were intended to be single crystals of these compounds, making it difficult to interpret bulk property measurements. Here, we use a combination of two advanced microscopy techniques to provide direct evidence of the magnetic properties of the individual phases. First, x-ray linear dichroism studies in a photoelectron emission microscope, and supporting multiplet calculations, indicate that the matrix (majority) phase is antiferromagnetic whereas the minority phase is nonmagnetic at room temperature. Second, cryogenic magnetic force microscopy demonstrates unambiguously that superconductivity occurs only in the minority phase. The correlation of these findings with previous microstructural studies and bulk measurements paves the way for understanding the intriguing electronic and magnetic
ZERO-FIELD NUCLEAR MAGNETIC RESONANCE FOR STUDY OF ANTIFERROMAGNETIC PROPERTIES OF FeF3 MATERIALS
Directory of Open Access Journals (Sweden)
G. R. F. Suwandi
2016-01-01
Full Text Available Nuclear Magnetic Resonance (NMR has been used as a research tool in many fields. In this study, the magnetic properties, especially anti-ferromagnetic properties of FeF3 materials were investigated. Zero-field custom-built NMR method was used to investigate the anti-ferromagnetic properties in the materials. Experiments have been carried out by varying the sample temperatures from 8 K to 220 K. Ordinary spin echo pulse sequence 90⁰RF–τ–180⁰RF were used. Using Fast Fourier Transform, the signals in NMR spectrum were analyzed and the peak showed the resonance frequency. The result showed that resonance frequencies decrease with increasing in temperature. The frequency of the spectrum was around 85.41 MHz in the zero-temperature limit, and this corresponds with Fe hyperfine field at zero-temperature limit was 2.14 T. The temperature dependence of the local magnetization does not fit T2 Bloch’s Law very well. Instead, it fits the exponential form having an energy gap in the dispersion relation of the spin wave. It is obtained from the result that FeF3 is antiferromagnetic materials with energy gap of 11.466 meV and anisotropy energy of 1.045 meV.Nuclear Magnetic Resonance (NMR telah banyak digunakan sebagai “research tool” pada berbagai bidang kajian di fisika. Pada studi ini, akan dilakukan eksperimen untuk menguji sifat magnetik, khususnya antiferromagnetik pada material FeF3. Telah dilakukan eksperimen dengan memvariasikan temperatur pada sampel dari 8 K hingga 220 K. Pulse sequence yang digunakan adalah 90⁰RF–τ–180⁰RF. Dengan memanfaatkan Fast Fourier Transform, sinyal echo ini dapat dianalisis dalam bentuk spektrum NMR dengan puncak spektrum menunjukkan frekuensi resonansinya. Diperoleh bahwa frekuensi resonansi akan menurun seiring dengan kenaikan temperatur. Posisi frekuensi pada temperatur 0 K adalah sebesar 85,41 MHz, hal ini memperlihatkan bahwa medan hyperfine dari Fe sebesar 2,14 T pada temperatur 0 K. Kurva
International Nuclear Information System (INIS)
Sergeicheva, E. G.; Sosin, S. S.; Prozorova, L. A.; Gu, G. D.; Zaliznyak, I. A.
2017-01-01
We report on an electron spin resonance (ESR) study of a nearly one-dimensional (1D) spin-1/2 chain antiferromagnet, Sr 2 CuO 3 , with extremely weak magnetic ordering. The ESR spectra at T > T N , in the disordered Luttinger-spin-liquid phase, reveal nearly ideal Heisenberg-chain behavior with only a very small, field-independent linewidth, ~1/T. In the ordered state, below T N , we identify field-dependent antiferromagnetic resonance modes, which are well described by pseudo-Goldstone magnons in the model of a collinear biaxial antiferromagnet. Additionally, we observe a major resonant mode with unusual and strongly anisotropic properties, which is not anticipated by the conventional theory of Goldstone spin waves. Lastly, we propose that this unexpected magnetic excitation can be attributed to a field-independent magnon mode renormalized due to its interaction with the high-energy amplitude (Higgs) mode in the regime of weak spontaneous symmetry breaking.
Transport and magnetic properties of new heavy-fermion antiferromagnet YbNi{sub 3}Al{sub 9}
Energy Technology Data Exchange (ETDEWEB)
Ohara, S; Yamashita, T; Mori, Y; Sakamoto, I, E-mail: ohara.shigeo@nitech.ac.jp [Department of Engineering Physics, Electronics and Mechanics, Graduate School of Engineering, Nagoya Institute of Technology, Nagoya 466-8555 (Japan)
2011-01-01
We have synthesized a new Yb-based Kondo-lattice compound YbNi{sub 3}Al{sub 9}. This compound crystallizes in a trigonal ErNi{sub 3}Al{sub 9}-type structure (space group R32), in which the Yb-ion is arranged in a two-dimensional honey-comb lattice perpendicular to the c-axis. We report the first measurements of electrical resistivity and magnetization for single-crystalline samples of YbNi{sub 3}Al{sub 9}. The electrical resistivity of YbNi{sub 3}Al{sub 9} is characteristic of the typical properties of heavy-fermion antiferromagnets with a Neel temperature of T{sub N} = 3.4 K. The transport and magnetic properties exhibit large anisotropy in the low-temperature region owing to an interplay among the crystalline-electric-field effect, the Ruderman-Kittel-Kasuya-Yoshida interaction, and the Kondo effect. Below T{sub N}, the metamagnetic transition is observed at a very low magnetic field of around 1 kOe with the field applied along the a-axis. The magnetic structure of YbNi{sub 3}Al{sub 9} is highly sensitive to the applied magnetic field.
Shao, Yangfan; Pang, Rui; Pan, Hui; Shi, Xingqiang
2018-03-01
The interfaces between organic molecules and magnetic metals have gained increasing interest for both fundamental reasons and applications. Among them, the C60/layered antiferromagnetic (AFM) interfaces have been studied only for C60 bonded to the outermost ferromagnetic layer [S. L. Kawahara et al., Nano Lett. 12, 4558 (2012) and D. Li et al., Phys. Rev. B 93, 085425 (2016)]. Here, via density functional theory calculations combined with evidence from the literature, we demonstrate that C60 adsorption can reconstruct the layered-AFM Cr(001) surface at elevated annealing temperatures so that C60 bonds to both the outermost and the subsurface Cr layers in opposite spin directions. Surface reconstruction drastically changes the adsorbed molecule spintronic properties: (1) the spin-split p-d hybridization involves multi-orbitals of C60 and top two layers of Cr with opposite spin-polarization, (2) the subsurface Cr atom dominates the C60 electronic properties, and (3) the reconstruction induces a large magnetic moment of 0.58 μB in C60 as a synergistic effect of the top two Cr layers. The induced magnetic moment in C60 can be explained by the magnetic direct-exchange mechanism, which can be generalized to other C60/magnetic metal systems. Understanding these complex hybridization behaviors is a crucial step for molecular spintronic applications.
Kagesawa, Koichi; Nishimura, Yuki; Yoshida, Hiroki; Breedlove, Brian K; Yamashita, Masahiro; Miyasaka, Hitoshi
2017-03-07
Two-dimensional layered compounds with different counteranions, [{Mn(salen)} 4 C6](BF 4 ) 2 ·2(CH 3 OH) (1) and [{Mn(salen)} 4 C6](PF 6 ) 2 ·2(CH 3 OH) (2) (salen 2- = N,N'-bis(salicylideneiminato), C6 2- = C 6 H 12 (COO) 2 2- ), were synthesized by assembling [Mn(salen)(H 2 O)]X (X - = BF 4 - and PF 6 - ) and C 6 H 12 (CO 2 - ) 2 (C6 2- ) in a methanol/2-propanol medium. The compounds have similar structures, which are composed of Mn(salen) out-of-plane dimers bridged by μ 4 -type C6 2- ions, forming a brick-wall-type network of [-{Mn 2 }-OCO-] chains alternately connected via C 6 H 12 linkers of C6 2- moieties. The counteranions for 1 and 2, i.e., BF 4 - and PF 6 - , respectively, are located between layers. Since the size of BF 4 - is smaller than that of PF 6 - , intra-layer inter-chain and inter-plane nearest-neighbor MnMn distances are shorter in 1 than in 2. The zigzag chain moiety of [-{Mn 2 }-OCO-] leads to a canted S = 2 spin arrangement with ferromagnetic coupling in the Mn III out-of-plane dimer moiety and antiferromagnetic coupling through -OCO- bridges. Due to strong uniaxial anisotropy of the Mn III ion, the [-{Mn 2 }-OCO-] chains could behave as a single-chain magnet (SCM), which exhibits slow relaxation of magnetization at low temperatures. Nevertheless, these compounds fall into an antiferromagnetic ground state at higher temperatures of T N = 4.6 and 3.8 K for 1 and 2, respectively, than active temperatures for SCM behavior. The spin flip field at 1.8 K is 2.7 and 1.8 kOe for 1 and 2, respectively, which is attributed to the inter-chain interactions tuned by the size of the counteranions. The relaxation times of magnetization become longer at the boundary between the antiferromagnetic phase and the paramagnetic phase.
Quasi one dimensional transport in individual electrospun composite nanofibers
Energy Technology Data Exchange (ETDEWEB)
Avnon, A., E-mail: avnon@phys.fu-berlin.de; Datsyuk, V.; Trotsenko, S. [Institut für Experimentalphysik, Freie Universität Berlin, Arnimallee 14, 14195 Berlin (Germany); Wang, B.; Zhou, S. [Research Center of Microperipheric Technologies, Technische Universität Berlin, TiB4/2-1, Gustav-Meyer-Allee 25, 13355 Berlin (Germany); Grabbert, N.; Ngo, H.-D. [Microsystem Engineering (FB I), University of Applied Sciences, Wilhelminenhofstr. 74 (C 525), 12459 Berlin (Germany)
2014-01-15
We present results of transport measurements of individual suspended electrospun nanofibers Poly(methyl methacrylate)-multiwalled carbon nanotubes. The nanofiber is comprised of highly aligned consecutive multiwalled carbon nanotubes. We have confirmed that at the range temperature from room temperature down to ∼60 K, the conductance behaves as power-law of temperature with an exponent of α ∼ 2.9−10.2. The current also behaves as power law of voltage with an exponent of β ∼ 2.3−8.6. The power-law behavior is a footprint for one dimensional transport. The possible models of this confined system are discussed. Using the model of Luttinger liquid states in series, we calculated the exponent for tunneling into the bulk of a single multiwalled carbon nanotube α{sub bulk} ∼ 0.06 which agrees with theoretical predictions.
Investigation of quasi-one-dimensional finite phononic crystal with ...
Indian Academy of Sciences (India)
discrete models in the LM method, the increment of the number of components in a unit cell cannot ... frequency-response function (FRF) or transmission coefficients. The width of the .... where i is an integer and t is the discrete time interval.
Phonon scattering in quasi-one-dimensional structure
Energy Technology Data Exchange (ETDEWEB)
Bourahla, B., E-mail: bourahla_boualem@yahoo.f [Laboratoire de Physique et Chimie Quantique, Universite de Tizi Ouzou, BP 17 RP 15000 (Algeria); Laboratoire de Physique de l' etat Condense, UMR 6087, Universite du Maine, 72085 Le Mans (France); Nafa, O. [Laboratoire de Physique et Chimie Quantique, Universite de Tizi Ouzou, BP 17 RP 15000 (Algeria); Tigrine, R. [Laboratoire de Physique et Chimie Quantique, Universite de Tizi Ouzou, BP 17 RP 15000 (Algeria); Laboratoire de Physique de l' etat Condense, UMR 6087, Universite du Maine, 72085 Le Mans (France)
2011-02-15
We introduce a model to study a symmetric nanocontact, whereby its mechanical properties can be analyzed via the vibration spectra. The model system consists of two groups of triple semi-infinite atomic chains joined by atoms in between. The matching method theoretical approach is used to calculate the coherent reflection and transmission scattering probabilities, the characteristic vibration Green functions and densities of states (DOS), for the vibration components of the individual atomic sites that constitute a complete representation of the nanocontact domain boundaries. The nanocontact observables are numerically calculated for different cases of elastic hardening and softening, to investigate how the local dynamics can respond to changes in the microscopic environment on the nanocontact domain. The analysis of the vibration spectra and the DOS demonstrate the fluctuations, related to Fano resonances, due to the coherent coupling between traveling phonons and the localized vibration modes in the nanocontact domain.
Spin reorientation via antiferromagnetic coupling
Energy Technology Data Exchange (ETDEWEB)
Ranjbar, M., E-mail: mojtaba.ranjbar@physics.gu.se [Data Storage Institute, A-STAR (Agency for Science, Technology and Research), 5, Engineering Drive 1, Singapore 117608 (Singapore); Department of Physics, University of Gothenburg, 412 96 Gothenburg (Sweden); Sbiaa, R. [Data Storage Institute, A-STAR (Agency for Science, Technology and Research), 5, Engineering Drive 1, Singapore 117608 (Singapore); Department of Physics, Sultan Qaboos University, P.O. Box 36, PC 123, Muscat (Oman); Dumas, R. K. [Department of Physics, University of Gothenburg, 412 96 Gothenburg (Sweden); Åkerman, J. [Department of Physics, University of Gothenburg, 412 96 Gothenburg (Sweden); Materials Physics, School of ICT, Royal Institute of Technology (KTH), 164 40 Kista (Sweden); Piramanayagam, S. N. [Data Storage Institute, A-STAR (Agency for Science, Technology and Research), 5, Engineering Drive 1, Singapore 117608 (Singapore)
2014-05-07
Spin reorientation in antiferromagnetically coupled (AFC) Co/Pd multilayers, wherein the thickness of the constituent Co layers was varied, was studied. AFC-Co/Pd multilayers were observed to have perpendicular magnetic anisotropy even for a Co sublayer thickness of 1 nm, much larger than what is usually observed in systems without antiferromagnetic coupling. When similar multilayer structures were prepared without antiferromagnetic coupling, this effect was not observed. The results indicate that the additional anisotropy energy contribution arising from the antiferromagnetic coupling, which is estimated to be around 6 × 10{sup 6} ergs/cm{sup 3}, induces the spin-reorientation.
DEFF Research Database (Denmark)
Jiang, Jianzhong; Mørup, Steen
1997-01-01
The influence of the particle size distribution on the ratio of the peak temperature, T-peak, to the blocking temperature, T-Bm, in zero field cooled (ZFD) magnetization curves has studied for both ferromagnetic and antiferromagnetic particle systems. In both systems the ratio beta=T-peak/T-Bm does...... not depend on the median particle volume. However, T-Bm can be considerably different from T-peak in both systems. These results show that the ZFD measurements can be used to determine T-Bm values only if the particle size distribution of the system is known. Otherwise, the estimated T-Bm values will have...... a large uncertainty, especially in systems with a broad particle size distribution....
International Nuclear Information System (INIS)
Zeng, Z.; Duan, Y.; Guenzburger, Diana
1996-09-01
The electronic and magnetic properties of the nanometer-size antiferromagnet (the ferric wheel molecule) are investigated with the first-principles spin-polarized Discrete Variational Method, in the framework of Density Functional theory. Magnetic moments, densities of the states and charge and spin-density maps are obtained. The Moessbauer hyperfine parameters Isomer shift, Quadrupole Splitting and Hyperfine Field are obtained from the calculations and compared to reported experimental values when available. (author). 33 refs., 8 figs., 4 tabs
Jungwirth, T.
2017-05-30
This focused issue attempts to provide a comprehensive introduction into the field of antiferromagnetic spintronics. Apart from the brief overview below, it features five review articles. The intention is to cover in a coherent and complementary way key physical aspects of the antiferromagnetic spintronics research. These range from microelectronic memory devices and optical manipulation and detection of antiferromagnetic spins, to the fundamentals of antiferromagnetic dynamics in uniform or spin-textured systems, and to the interplay of antiferromagnetic spintronics with topological phenomena. The antiferromagnetic ordering can take a number of forms including fully compensated collinear, non-collinear, and non-coplanar magnetic lattices, compensated and uncompensated ferrimagnets, or metamagnetic materials hosting an antiferromagnetic to ferromagnetic phase transition. Apart from the variety of distinct magnetic crystal structures, the focused issue also encompasses spintronic phenomena and devices studied in antiferromagnet/ferromagnet heterostructures and in synthetic antiferromagnets.
Jungwirth, T.; Sinova, J.; Manchon, Aurelien; Marti, X.; Wunderlich, J.; Felser, C.
2017-01-01
This focused issue attempts to provide a comprehensive introduction into the field of antiferromagnetic spintronics. Apart from the brief overview below, it features five review articles. The intention is to cover in a coherent and complementary way key physical aspects of the antiferromagnetic spintronics research. These range from microelectronic memory devices and optical manipulation and detection of antiferromagnetic spins, to the fundamentals of antiferromagnetic dynamics in uniform or spin-textured systems, and to the interplay of antiferromagnetic spintronics with topological phenomena. The antiferromagnetic ordering can take a number of forms including fully compensated collinear, non-collinear, and non-coplanar magnetic lattices, compensated and uncompensated ferrimagnets, or metamagnetic materials hosting an antiferromagnetic to ferromagnetic phase transition. Apart from the variety of distinct magnetic crystal structures, the focused issue also encompasses spintronic phenomena and devices studied in antiferromagnet/ferromagnet heterostructures and in synthetic antiferromagnets.
Prospect for antiferromagnetic spintronics
Czech Academy of Sciences Publication Activity Database
Martí, Xavier; Fina, I.; Jungwirth, Tomáš
2015-01-01
Roč. 51, č. 4 (2015), s. 2900104 ISSN 0018-9464 R&D Projects: GA MŠk(CZ) LM2011026; GA ČR GB14-37427G EU Projects: European Commission(XE) 268066 - 0MSPIN Institutional support: RVO:68378271 Keywords : spintronics * antiferromagnets Subject RIV: BM - Solid Matter Physics ; Magnetism Impact factor: 1.277, year: 2015
Energy Technology Data Exchange (ETDEWEB)
Nuss, Juergen; Jansen, Martin [Max-Planck-Institut fuer Festkoerperforschung, Stuttgart (Germany); Senaris-Rodriguez, Maria A. [Dept. Quimica, Facultad de Ciencias, Universidad de A Coruna (Spain); Klemenz, Sebastian [Max-Planck-Institut fuer Chemische Physik fester Stoffe, Dresden (Germany)
2017-11-17
Cs{sub 23}Mn{sub 16}O{sub 23} was synthesized via the azide/nitrate route from mixtures of Mn{sub 2}O{sub 3}, CsNO{sub 3}, and CsN{sub 3}. This manganese(II/III) mixed-valent oxide, which contains only one Mn{sup 3+} besides 15 Mn{sup 2+} cations, was studied by single-crystal X-ray diffraction and magnetic susceptibility measurements. Its crystal structure [P anti 1, Z = 1, a = 1114.26(2), b = 1185.53(2), c = 1205.39(2) pm, α = 70.596(1), β = 80.377(2), γ = 83.072(2) , R{sub 1} = 0.033] is based on a honeycomb-like arrangement of cesium atoms, providing the space for two different types of one-dimensional polyoxomanganate anions, illustrated by the syntax Cs{sub 23}[MnO{sub 2}]{sub 4}[Mn{sub 3}O{sub 5}]{sub 4}. Magnetic susceptibility measurements indicate dominant antiferromagnetic intra-chain interactions present already at ambient temperature and long range inter-chain magnetic ordering at 11 K. (copyright 2017 WILEY-VCH Verlag GmbH and Co. KGaA, Weinheim)
Bhowmik, R. N.; Venkata Siva, K.; Ranganathan, R.; Mazumdar, Chandan
2017-06-01
The samples of Ga-doped Cr2O3 have been prepared using chemical co-precipitation route. X-ray diffraction pattern and Raman spectra have indicated rhombohedral crystal structure with space group R 3 bar C. Magnetic measurements indicated diluted antiferromagnetic (AFM) spin order in Ga-doped α-Cr2O3 and ferrimagnetic ordering of spins at about 50-60 K is confirmed from the analysis of the temperature dependence of dc magnetization and ac susceptibility data. Apart from magnetic dilution effect, the samples have shown superparamagnetic behavior below 50 K due to frustrated surface spins of the nano-sized grains. The samples have shown non-linear electronic properties. The current-voltage (I-V) characteristics of the Ga-doped α-Cr2O3 samples are remarkably different from α-Cr2O3 sample. The bi-stable electronic states and negative differential resistance are some of the unique non-linear electronic properties that the I-V curves of Ga-doped samples have exhibited. Optical study revealed three electronic transitions in the samples associated with band gap energy at about 2.67-2.81 eV, 1.91-2.11 eV, 1.28-1.35 eV, respectively. The results indicated multi-level electronic structure in Ga-doped α-Cr2O3 system.
Magnetic properties of S=l/2 antiferromagnetic XXZ model on the Shastry-Sutherland lattices
International Nuclear Information System (INIS)
Suzuki, Takafumi; Tomita, Yusuke; Kawashima, Naoki
2010-01-01
We study magnetic properties of the S=l/2 Ising-like XXZ model on the Shastry-Sutherland lattices considering the effect of long range interactions. By performing quantum Monte Carlo simulations, we find that magnetization plateau phases appear at one-half and one-third of the saturation magnetization. We also study the finite temperature transition to the magnetic plateau phases and discuss the universality class of the transition.
Electronic and magnetic properties of organic conductors (DMET)2MBr4 (M=Fe, Ga)
International Nuclear Information System (INIS)
Enomoto, Kengo; Miyazaki, Akira; Enoki, Toshiaki; Yamaura, Jun-ichi
2003-01-01
(DMET) 2 MBr 4 (M=Fe, Ga) are isostructural organic conductors whose crystal structure consists of an alternate stacking of quasi one-dimensional chain-based donor layers and anion square lattices. The resistivity, ESR, magnetic susceptibility, magnetization, and magnetoresistance of these salts were investigated in order to clarify the correlation between the electronic structure and the magnetism. The electronic structures of both salts are metallic down to T MI - 40 K, below which a Mott insulating state is stabilized, accompanied by an SDW transition at T SDW - 25 K. The FeBr 4 salt with Fe 3+ (S=5/2) localized spins undergoes an antiferromagnetic transition at T N = 3.7 K. In the FeBr 4 salt, the magnetization curves, which show field-direction-dependent anomalies in addition to a spin-flop transition, are demonstrated to have a participation of donor π-electron spins in the magnetization processes. The field dependence of the magnetoresistances below T N tracks faithfully that of the magnetization, where the donor π-electrons and Fe 3+ d-electrons are responsible for the former and the latter, respectively. This clearly demonstrates the presence of the π-d interaction that plays an important role in the interplay between electron transport and magnetism. (author)
Energy Technology Data Exchange (ETDEWEB)
Tian, Yong; Kong, Yixiu; Liu, Kai; Zhang, Anmin [Department of Physics, Beijing Key Laboratory of Opto-electronic Functional Materials & Micro-nano Devices, Renmin University of China, Beijing 100872 (China); He, Rui [Department of Physics, University of Northern Iowa, Cedar Falls, Iowa 50614 (United States); Zhang, Qingming, E-mail: qmzhang@ruc.edu.cn [Department of Physics, Beijing Key Laboratory of Opto-electronic Functional Materials & Micro-nano Devices, Renmin University of China, Beijing 100872 (China)
2017-05-01
ThCr{sub 2}Si{sub 2}-type phosphide ACo{sub 2}P{sub 2} (A=Eu, La, Pr, Nd, Ce) has the same structure as iron arsenides, but their magnetic behaviors are quite distinct. In this paper, we grew a series of La{sub 1−x}Ce{sub x}Co{sub 2}P{sub 2} single crystals (x=0.0 to1.0), made structural and magnetic characterizations. We found the introduction of cerium induces a rapid decrease of c-axis and a change from ferromagnetic to antiferromagnetic states. Compared to other trivalent doped compounds, the enhancement of ferromagnetism with doping is suppressed and the transition from ferromagnetism to antiferromagnetism appear earlier. By employing first-principles band-structure calculations, we identify the increase of Ce valence suppress the itinerant ferromagnetism and leading to formation of P-P bonding with the shortening of c-axis. The bonding effectively drives an increase of interlayer antiferromagnetic interaction, eventually leads to antiferromagnetic ordering of cobalt in high-doping region.
Study of synthetic ferrimagnet-synthetic antiferromagnet structures for magnetic sensor application
Guedes, A.; Mendes, M. J.; Freitas, P. P.; Martins, J. L.
2006-04-01
There has been a growing interest in using both synthetic ferrimagnet (SF) free and synthetic antiferromagnet (SAF) pinned layers for head and memory applications. In particular, for linear sensor applications, these structures lower the magnetostatic fields present at the free layer through the reduction of its effective thickness (teffSF). This allows higher sensitivity but at the expense of an increased offset field H0(Néel coupling field Hf+interlayer demagnetizing field HdSAF). In this work, results on a series of patterned 3×1 and 6×2 μm2 top-pinned SF-SAF spin valves are analyzed and compared with a three-dimensional micromagnetic simulation in order to clarify the role of the different ferromagnetic layers in the overall offset field and sensitivity. H0 varies as 1/teffSF[teffSF=(Mata-Mbtb)/MeffSF]. The magnetostatic field acting on the SF coming from the SAF (HdSAF) can act as a biasing field, partially counterbalancing the Néel coupling field (Hf) leading to a reduction of H0. In this work the offset field was reduced from an initial value of 25 Oe in a quasicompensated SAF to a value of -6 Oe, by unbalancing the SAF and consequently increasing its effective moment (teffSF=15 A˚).
Energy Technology Data Exchange (ETDEWEB)
Loeffler, J.; Wagner, W. [Paul Scherrer Inst. (PSI), Villigen (Switzerland); Kostorz, G. [Eidgenoessische Technische Hochschule, Zurich (Switzerland); Wiedenmann, A. [HMI Berlin (Germany)
1997-09-01
Magnetic small-angle neutron scattering measurements were performed on nanostructured ferromagnetic materials on the basis of Fe, Ni and Co, produced preferentially by the inert-gas condensation technique, with the aim to determine the magnetic microstructure of mesoscopic small-particle systems. (author) 1 fig., 3 refs.
Magnetic dichroism and spin structure of antiferromagnetic NiO(001) films
Altieri, S; Finazzi, M; Hsieh, HH; Lin, HJ; Chen, CT; Hibma, T; Valeri, S; Sawatzky, GA
2003-01-01
We find that Ni L-2 edge x-ray magnetic linear dichroism is fully reversed for NiO(001) films on materials with reversed lattice mismatch. We relate this phenomenon to a preferential stabilization of magnetic S domains with main spin component either in or out of the plane, via dipolar interactions.
Spin model for nontrivial types of magnetic order in inverse-perovskite antiferromagnets
Mochizuki, Masahito; Kobayashi, Masaya; Okabe, Reoya; Yamamoto, Daisuke
2018-02-01
Nontrivial magnetic orders in the inverse-perovskite manganese nitrides are theoretically studied by constructing a classical spin model describing the magnetic anisotropy and frustrated exchange interactions inherent in specific crystal and electronic structures of these materials. With a replica-exchange Monte Carlo technique, a theoretical analysis of this model reproduces the experimentally observed triangular Γ5 g and Γ4 g spin-ordered patterns and the systematic evolution of magnetic orders. Our Rapid Communication solves a 40-year-old problem of nontrivial magnetism for the inverse-perovskite manganese nitrides and provides a firm basis for clarifying the magnetism-driven negative thermal expansion phenomenon discovered in this class of materials.
The magnetic state of diamagnetically diluted antiferromagnetic cobalt and nickel monoxide
International Nuclear Information System (INIS)
Masrour, R.; Hamedoun, M.; Benyoussef, A.
2009-01-01
The nearest neighbour J 1 (x) and the next-neighbour super-exchange J 2 (x) interactions are evaluated by using the mean field theory for Mg 1-x B x O (B=Co and Ni) systems. The magnetic energy E(x) is obtained. A magnetic phase diagram of the Mg 1-x B x O (B=Co and Ni) solid solutions with 0≤x≤1 is drawn by high-temperature series expansions (HTSE) combined with the Pade approximants method (PA). The critical exponents associated with the magnetic susceptibility (γ) and with the correlation length (ν) are deduced in order phase.
Crystal structure and magnetic properties of the Cr-doped spiral antiferromagnet BiMnFe2O6
International Nuclear Information System (INIS)
Batuk, Dmitry; De Dobbelaere, Christopher; Tsirlin, Alexander A.; Abakumov, Artem M.; Hardy, An; Van Bael, Marlies K.; Greenblatt, Martha; Hadermann, Joke
2013-01-01
Graphical abstract: - Highlights: • The substitution of Cr for Mn in BiMnFe 2 O 6 is possible by the solution–gel method. • The BiCr x Mn 1−x Fe 2 O 6 solid solution is obtained for the x values up to 0.3. • Increasing Cr content lowers the temperature of the antiferromagnetic ordering. - Abstract: We report the Cr 3+ for Mn 3+ substitution in the BiMnFe 2 O 6 structure. The BiCr x Mn 1−x Fe 2 O 6 solid solution is obtained by the solution–gel synthesis technique for the x values up to 0.3. The crystal structure investigation using a combination of X-ray powder diffraction and transmission electron microscopy demonstrates that the compounds retain the parent BiMnFe 2 O 6 structure (for x = 0.3, a = 5.02010(6)Å, b = 7.06594(7)Å, c = 12.6174(1)Å, S.G. Pbcm, R I = 0.036, R P = 0.011) with only a slight decrease in the cell parameters associated with the Cr 3+ for Mn 3+ substitution. Magnetic susceptibility measurements suggest strong similarities in the magnetic behavior of BiCr x Mn 1−x Fe 2 O 6 (x = 0.2; 0.3) and parent BiMnFe 2 O 6 . Only T N slightly decreases upon Cr doping that indicates a very subtle influence of Cr 3+ cations on the magnetic properties at the available substitution rates
Energy Technology Data Exchange (ETDEWEB)
Adelnia, Fatemeh [Dipartimento di Fisica, Università degli Studi di Milano and INSTM, I-20133 Milano (Italy); Dipartimento di Fisica, Università degli Studi di Pavia and INSTM, I-27100 Pavia (Italy); Chiesa, Alessandro; Bordignon, Sara; Carretta, Stefano [Dipartimento di Fisica e Scienze della Terra, Università degli Studi di Parma, I-43124 Parma (Italy); Ghirri, Alberto; Candini, Andrea [CNR Institute Nanosciences S3, I- 41125 Modena (Italy); Cervetti, Christian [Dipartimento di Scienze Fisiche, Informatiche, Matematiche, Università di Modena e Reggio Emilia, I-41125 Modena (Italy); Evangelisti, Marco [CNR Institute Nanosciences S3, I- 41125 Modena (Italy); Dipartimento di Scienze Fisiche, Informatiche, Matematiche, Università di Modena e Reggio Emilia, I-41125 Modena (Italy); Instituto de Ciencia de Materiales de Aragón and Departamento de Física de la Materia Condensada, CSIC-Universidad de Zaragoza, 50009 Zaragoza (Spain); Affronte, Marco [CNR Institute Nanosciences S3, I- 41125 Modena (Italy); Dipartimento di Scienze Fisiche, Informatiche, Matematiche, Università di Modena e Reggio Emilia, I-41125 Modena (Italy); Sheikin, Ilya [Grenoble High Magnetic Field Laboratory, CNRS-LNCMI, 25, B.P. 166, 38042 Grenoble Cedex 9 (France); Winpenny, Richard; Timco, Grigore [The Lewis Magnetism Laboratory, The University of Manchester, M13 9PL Manchester (United Kingdom); Borsa, Ferdinando [Dipartimento di Fisica, Università degli Studi di Pavia and INSTM, I-27100 Pavia (Italy); and others
2015-12-28
A detailed experimental investigation of the effects giving rise to the magnetic energy level structure in the vicinity of the level crossing (LC) at low temperature is reported for the open antiferromagnetic molecular ring Cr{sub 8}Zn. The study is conducted by means of thermodynamic techniques (torque magnetometry, magnetization and specific heat measurements) and microscopic techniques (nuclear magnetic resonance line width, nuclear spin lattice, and spin-spin relaxation measurements). The experimental results are shown to be in excellent agreement with theoretical calculations based on a minimal spin model Hamiltonian, which includes a Dzyaloshinskii-Moriya interaction. The first ground state level crossing at μ{sub 0}H{sub c1} = 2.15 T is found to be an almost true LC while the second LC at μ{sub 0}H{sub c2} = 6.95 T has an anti-crossing gap of Δ{sub 12} = 0.19 K. In addition, both NMR and specific heat measurements show the presence of a level anti-crossing between excited states at μ{sub 0}H = 4.5 T as predicted by the theory. In all cases, the fit of the experimental data is improved by introducing a distribution of the isotropic exchange couplings (J), i.e., using a J strain model. The peaks at the first and second LCs in the nuclear spin-lattice relaxation rate are dominated by inelastic scattering and a value of Γ ∼ 10{sup 10} rad/s is inferred for the life time broadening of the excited state of the open ring, due to spin phonon interaction. A loss of NMR signal (wipe-out effect) is observed for the first time at LC and is explained by the enhancement of the spin-spin relaxation rate due to the inelastic scattering.
Field-induced phase transitions in antiferromagnetic systems
International Nuclear Information System (INIS)
Smeets, J.P.M.
1984-05-01
Neutron scattering experiments and magnetization measurements are carried out on cobalt bromide hexahydrate, of which 48% of the water molecules are replaced by deuterium oxide molecules. Results were compared with data obtained from non-deuterated cobalt bromide hexahydrate. Neutron scattering experiments showed the importance of the deuterium fraction. Interplay exists between the crystallographic system and the magnetic system, which is influenced by changing the deuterium fraction. Neutron scattering and magnetization experiments on partially deuterated RbFeCl 3 .2H 2 O and CsFeCl 3 .2H 2 O were performed to study the magnetic phase transitions in these quasi one-dimensional Ising compounds. The observed behaviour in the various phases can be described by the nucleation theory of chain reversals. (Auth.)
Electronic structure and magnetic ordering of the unconventional antiferromagnet Yb3Pt4
Schwingenschlögl, Udo
2009-12-01
Applying density functional theory within the generalized gradient approximation, we investigate the electronic and magnetic properties of the intermetallic rare-earth system Yb3Pt4. This material recently has been put forward as host for quantum criticality, while details of the magnetic ordering could not be established (Bennett N. C.et al., J. Magn. & Magn. Mater., 321 (2009) 2021). In this context, we investigate the effect of spin-orbit coupling and compare various spin patterns from the energetic point of view, which enables us to determine the electronic ground state of Yb3Pt4. The assumption of an elementary superexchange mechanism yields a magnetic-coupling constant in good agreement with the experimental ordering temperature. Copyright © 2009 EPLA.
Electronic structure and magnetic ordering of the unconventional antiferromagnet Yb3Pt4
Schwingenschlö gl, Udo; Gó mez, Javier Alexandra M; Grau-Crespo, Ricardo
2009-01-01
Applying density functional theory within the generalized gradient approximation, we investigate the electronic and magnetic properties of the intermetallic rare-earth system Yb3Pt4. This material recently has been put forward as host for quantum criticality, while details of the magnetic ordering could not be established (Bennett N. C.et al., J. Magn. & Magn. Mater., 321 (2009) 2021). In this context, we investigate the effect of spin-orbit coupling and compare various spin patterns from the energetic point of view, which enables us to determine the electronic ground state of Yb3Pt4. The assumption of an elementary superexchange mechanism yields a magnetic-coupling constant in good agreement with the experimental ordering temperature. Copyright © 2009 EPLA.
Czech Academy of Sciences Publication Activity Database
Gomonay, O.; Kläui, M.; Sinova, Jairo
2016-01-01
Roč. 109, č. 14 (2016), 1-4, č. článku 142404. ISSN 0003-6951 R&D Projects: GA ČR GB14-37427G Institutional support: RVO:68378271 Keywords : spintronics * solitons * Mn 2 Au Subject RIV: BM - Solid Matter Physics ; Magnetism Impact factor: 3.411, year: 2016
Concepts of antiferromagnetic spintronics
Czech Academy of Sciences Publication Activity Database
Gomonay, O.; Jungwirth, Tomáš; Sinova, Jairo
2017-01-01
Roč. 11, č. 4 (2017), 1-8, č. článku 1700022. ISSN 1862-6254 R&D Projects: GA MŠk LM2015087; GA ČR GB14-37427G Institutional support: RVO:68378271 Keywords : spintronics * antiferromagnets Subject RIV: BM - Solid Matter Physics ; Magnetism OBOR OECD: Condensed matter physics (including formerly solid state physics, supercond.) Impact factor: 3.032, year: 2016
μSR Study of the Unusual Magnetic Ordering in the Frustrated Antiferromagnet Zn(CrxGa1-x)2O4
International Nuclear Information System (INIS)
Kikuchi, H.; Fukushima, H.; Higemoto, W.; Nishiyama, K.
2001-01-01
μSR spectra on the spin frustrating spinel antiferromagnet Zn(Cr x Ga 1-x ) 2 O 4 (x=0.9,1.0) have been measured. For x=1.0 compound, both the relaxation rate and the initial asymmetry showed distinct anomalies at the Neel temperature. The magnetic susceptibility for the x=0.9 compound was known to have a faint peak at around 12 K, whose origin was not clear so far. Our μSR study revealed that this temperature is the onset temperature of development of the magnetic correlation accompanied by appreciable spin fluctuations.
Electronic and magnetic properties of organic conductors (DMET) sub 2 MBr sub 4 (M=Fe, Ga)
Enomoto, K; Enoki, T; Yamaura, J I
2003-01-01
(DMET) sub 2 MBr sub 4 (M=Fe, Ga) are isostructural organic conductors whose crystal structure consists of an alternate stacking of quasi one-dimensional chain-based donor layers and anion square lattices. The resistivity, ESR, magnetic susceptibility, magnetization, and magnetoresistance of these salts were investigated in order to clarify the correlation between the electronic structure and the magnetism. The electronic structures of both salts are metallic down to T sub M sub I - 40 K, below which a Mott insulating state is stabilized, accompanied by an SDW transition at T sub S sub D sub W - 25 K. The FeBr sub 4 salt with Fe sup 3 sup + (S=5/2) localized spins undergoes an antiferromagnetic transition at T sub N = 3.7 K. In the FeBr sub 4 salt, the magnetization curves, which show field-direction-dependent anomalies in addition to a spin-flop transition, are demonstrated to have a participation of donor pi-electron spins in the magnetization processes. The field dependence of the magnetoresistances below ...
Superconductivity in doped antiferromagnets
International Nuclear Information System (INIS)
Lagos, M.
1990-09-01
The antiferromagnetic S = 1/2 Heisenberg model is extended to account for the presence of holes. The holes move along a sublattice whose sites are located in between the spin sites. The spin-hole coupling arises from the modification of the exchange interaction between two neighbouring spins when the site between them is occupied by a hole. this physical picture leads to a generalized version of the so called t-J model Hamiltonian. The use of a recently developed method that introduces spin-O excitations for dealing with the Heisenberg antiferromagnetic model allows us to map the model Hamiltonian onto a Froelich one, with the spin-O magnetic excitations substituting phonons. The case of electrons moving along the spin sites is discussed as well. (author). 16 refs, 2 figs
Ramírez-Solís, A; Zicovich-Wilson, C M; Hernández-Lamoneda, R; Ochoa-Calle, A J
2017-01-25
The question of the non-magnetic (NM) vs. antiferromagnetic (AF) nature of the ε phase of solid oxygen is a matter of great interest and continuing debate. In particular, it has been proposed that the ε phase is actually composed of two phases, a low-pressure AF ε 1 phase and a higher pressure NM ε 0 phase [Crespo et al., Proc. Natl. Acad. Sci. U. S. A., 2014, 111, 10427]. We address this problem through periodic spin-restricted and spin-polarized Kohn-Sham density functional theory calculations at pressures from 10 to 50 GPa using calibrated GGA and hybrid exchange-correlation functionals with Gaussian atomic basis sets. The two possible configurations for the antiferromagnetic (AF1 and AF2) coupling of the 0 ≤ S ≤ 1 O 2 molecules in the (O 2 ) 4 unit cell were studied. Full enthalpy-driven geometry optimizations of the (O 2 ) 4 unit cells were done to study the pressure evolution of the enthalpy difference between the non-magnetic and both antiferromagnetic structures. We also address the evolution of structural parameters and the spin-per-molecule vs. pressure. We find that the spin-less solution becomes more stable than both AF structures above 50 GPa and, crucially, the spin-less solution yields lattice parameters in much better agreement with experimental data at all pressures than the AF structures. The optimized AF2 broken-symmetry structures lead to large errors of the a and b lattice parameters when compared with experiments. The results for the NM model are in much better agreement with the experimental data than those found for both AF models and are consistent with a completely non-magnetic (O 2 ) 4 unit cell for the low-pressure regime of the ε phase.
Wijngaard, Jan; Haas, C.; Groot, R.A. de
1992-01-01
Self-consistent spin-polarized energy-band calculations have been performed for Mn2Sb for a ferrimagnetic (FI), ferromagnetic (F), and antiferromagnetic (AF) spin alignment. The calculated local moments on the two types of Mn atoms are in agreement with values obtained from neutron diffraction for
Size effect on the magnetic properties of antiferromagnetic La0.2Ca0.8MnO3 nanoparticles
Markovich, V.; Fita, I.; Wisniewski, A.; Mogilyansky, D.; Puzniak, R.; Titelman, L.; Martin, C.; Gorodetsky, G.
2010-03-01
Magnetic properties of electron-doped La0.2Ca0.8MnO3 manganite nanoparticles with average particle size ranging from 15 to 37 nm, prepared by the glycine-nitrate method, have been investigated in temperature range 5-300 K and in magnetic fields up to 90 kOe. A monotonous enhancement of weak ferromagnetism linked to the reduction in the particle size was observed for all nanoparticles. Magnetic hysteresis loops also indicate size-dependent exchange bias effect displayed by horizontal and vertical shifts in field-cooled processes. The magnetization data reveal two ferromagnetic components: first one appears at T˜200K and may be attributed to surface magnetization and second one appears as a result of spin canting of antiferromagnetic core or is developed at some interfaces inside nanoparticles. Time evolution of magnetization recorded in magnetic fields after the field cooling to low temperatures exhibits a very noisy behavior that may be caused by formation of collective state of nanoparticles with no clear tendency to reach equilibrium state. Magnetic properties of the nanoparticle samples are compared with those of the bulk La0.2Ca0.8MnO3 .
Experimental and theoretical studies of nanoparticles of antiferromagnetic materials
DEFF Research Database (Denmark)
Mørup, Steen; Madsen, Daniel Esmarch; Frandsen, Cathrine
2007-01-01
The magnetic properties of nanoparticles of antiferromagnetic materials are reviewed. The magnetic structure is often similar to the bulk structure, but there are several examples of size-dependent magnetic structures. Owing to the small magnetic moments of antiferromagnetic nanoparticles, the co...
Diamond lattice Heisenberg antiferromagnet
Oitmaa, J.
2018-04-01
We investigate ground-state and high-temperature properties of the nearest-neighbour Heisenberg antiferromagnet on the three-dimensional diamond lattice, using series expansion methods. The ground-state energy and magnetization, as well as the magnon spectrum, are calculated and found to be in good agreement with first-order spin-wave theory, with a quantum renormalization factor of about 1.13. High-temperature series are derived for the free energy, and physical and staggered susceptibilities for spin S = 1/2, 1 and 3/2, and analysed to obtain the corresponding Curie and Néel temperatures.
Shore, Joel D.; Thurston, George M.
2018-01-01
We report a charge-patterning phase transition on two-dimensional square lattices of titratable sites, here regarded as protonation sites, placed in a low-dielectric medium just below the planar interface between this medium and a salt solution. We calculate the work-of-charging matrix of the lattice with use of a linear Debye-Hückel model, as input to a grand-canonical partition function for the distribution of occupancy patterns. For a large range of parameter values, this model exhibits an approximate inverse cubic power-law decrease of the voltage produced by an individual charge, as a function of its in-lattice separation from neighboring titratable sites. Thus, the charge coupling voltage biases the local probabilities of proton binding as a function of the occupancy of sites for many neighbors beyond the nearest ones. We find that even in the presence of these longer-range interactions, the site couplings give rise to a phase transition in which the site occupancies exhibit an alternating, checkerboard pattern that is an analog of antiferromagnetic ordering. The overall strength W of this canonical charge coupling voltage, per unit charge, is a function of the Debye length, the charge depth, the Bjerrum length, and the dielectric coefficients of the medium and the solvent. The alternating occupancy transition occurs above a curve of thermodynamic critical points in the (pH-pK,W) plane, the curve representing a charge-regulation analog of variation of the Néel temperature of an Ising antiferromagnet as a function of an applied, uniform magnetic field. The analog of a uniform magnetic field in the antiferromagnet problem is a combination of pH-pK and W, and 1/W is the analog of the temperature in the antiferromagnet problem. We use Monte Carlo simulations to study the occupancy patterns of the titratable sites, including interactions out to the 37th nearest-neighbor category (a distance of 74 lattice constants), first validating simulations through
International Nuclear Information System (INIS)
Pedro, I de; Rojo, J M; Pizarro, J L; Fernandez, J RodrIguez; Marcos, J Sanchez; Fernandez-DIaz, M T; Arriortua, M I; Rojo, T
2006-01-01
Compounds of the general formula Co 2-x Ni x (OH)PO 4 (x = 0.1, 0.3) have been synthesized under mild hydrothermal conditions. Neutron powder diffraction, susceptibility and heat capacity measurements were carried out on polycrystalline samples. The cobalt-nickel compounds are ordered as three-dimensional antiferromagnets with ordering temperatures of 70 and 64 K for x = 0.1 and x = 0.3, respectively. The magnetic study shows a spin glass-like state below 11 and 5 K for Co 1.9 Ni 0.1 (OH)PO 4 and Co 1.7 Ni 0.3 (OH)PO 4 , respectively. Specific heat data present peaks at 68 and 61 K for Co 1.9 Ni 0.1 and Co 1.7 Ni 0.3 , respectively. These peaks show broad shoulders between approximately 15 and 40 K. The lack of any distinguishable anomaly below 10 K supports the spin glass nature of the low temperature transitions. Refinement of room temperature neutron diffraction data indicates that the Ni(II) ions are in octahedral co-ordination with the practical absence of these ions in the trigonal bipyramidal sites. The magnetic structures of Co 2-x Ni x (OH)PO 4 consist of ferromagnetic arrangements between the octahedral chains and trigonal bipyramidal dimers within the xz plane with the magnetic moments along the z axis. The ferromagnetic layers are disposed antiparallel to one another along the y direction establishing the three-dimensional antiferromagnetic order (T N ∼70 K for Co 1.9 Ni 0.1 and ∼64 K for Co 1.7 Ni 0.3 ). The different exchange pathways, the anisotropy of the Co(II) ions and the frustration of the magnetic moments in the trigonal bipyramidal geometry could be responsible for the freezing process
International Nuclear Information System (INIS)
Wang Xiguang; Guo Guanghua; Zhang Guangfu
2011-01-01
The demagnetization processes of antiferromagnetically exchange-coupled hard/soft/hard trilayer structures have been studied based on the discrete one-dimensional atomic chain model and the linear partial domain-wall model. It is found that, when the magnetic anisotropy of soft layer is taken into account, the changes of the soft layer thickness and the interfacial exchange coupling strength may lead a transition of demagnetization process in soft layer from the reversible to the irreversible magnetic exchange-spring process. For the trilayer structures with very thin soft layer, the demagnetization process exhibits typical reversible exchange-spring behavior. However, as the thickness of soft layer is increased, there is a crossover point t c , after which the process becomes irreversible. Similarly, there is also a critical interfacial exchange coupling constant A sh c , above which the exchange-spring process is reversible. When A sh sh c , the irreversible exchange-spring process is achieved. The phase diagram of reversible and irreversible exchange-spring processes is mapped in the plane of the interfacial exchange coupling A sh and soft layer thickness N s . - Research highlights: → A differing magnetic exchange-spring process is found in antiferromagnetically exchange-coupled hard/soft/hard trilayers if the magnetic anisotropy of the soft layers is taken into account. → The change of the soft layer thickness may lead to a transition of demagnetization process in soft layer from the reversible to the irreversible exchange-spring process. → The change of the soft-hard interfacial exchange coupling strength may lead a transition of demagnetization process in soft layer from the reversible to the irreversible exchange-spring process. → The phase diagram of reversible and irreversible exchange-spring processes is mapped in the plane of the interfacial exchange coupling and soft layer thickness.
Magnetic properties of a S = 1/2 zigzag spin chain compound (N sub 2 H sub 5)CuCl sub 3
Maeshima, N; Narumi, Y; Kindo, K; Kobayashi, T C; Okunishi, K
2003-01-01
We present a theoretical and experimental study of a quasi-one-dimensional zigzag antiferromagnet (N sub 2 H sub 5)CuCl sub 3 , which can be viewed as weakly coupled Heisenberg chains with a frustrated interaction. We first discuss generic features of the magnetic properties of the zigzag spin chain between the nearly single chain case and the nearly double chain case, on the basis of the finite temperature density-matrix renormalization group (DMRG) calculations. We next show the experimental results for the magnetic susceptibility and the high-field magnetization of a single crystal of (N sub 2 H sub 5)CuCl sub 3 above the Neel temperature T sub N = 1.55 K. By comparing the experimental data with the DMRG results carefully, we finally obtain the ratio of the nearest and next-nearest exchange couplings as J sub 1 /J sub 2 = 0.25 with J sub 2 /k sub B = 16.3 K. We also investigate the three-dimensional (3D) coupling J' effect by using mean-field theory combined with the DMRG calculations. The estimated value ...
Energy Technology Data Exchange (ETDEWEB)
Franco, D.G.; Fuertes, V.C.; Blanco, M.C. [INFIQC (CONICET), Departamento de Fisicoquimica, Facultad de Ciencias Quimicas, Universidad Nacional de Cordoba, Ciudad Universitaria, X5000HUA Cordoba (Argentina); Fernandez-Diaz, M.T. [Institute Laue-Langevin (ILL) 156X, F-38042 Grenoble Cedex 9 (France); Sanchez, R.D., E-mail: rodo@cab.cnea.gov.ar [Centro Atomico Bariloche, CNEA and Instituto Balseiro, Universidad Nacional de Cuyo, Av. Bustillo 9500, 8400 Rio Negro (Argentina); Carbonio, R.E., E-mail: carbonio@fcq.unc.edu.ar [INFIQC (CONICET), Departamento de Fisicoquimica, Facultad de Ciencias Quimicas, Universidad Nacional de Cordoba, Ciudad Universitaria, X5000HUA Cordoba (Argentina)
2012-10-15
The synthesis, structural characterization, and magnetic properties of La{sub 3}Co{sub 2}SbO{sub 9} double perovskite are reported. The crystal structure has been refined by X-ray and neutron powder diffraction data in the monoclinic space group P2{sub 1}/n. Co{sup 2+} and Sb{sup 5+} have the maximum order allowed for the La{sub 3}Co{sub 2}SbO{sub 9} stoichiometry. Rietveld refinements of powder neutron diffraction data show that at room temperature the cell parameters are a=5.6274(2) A, b=5.6842(2) A, c=7.9748(2) A and {beta}=89.999(3) Degree-Sign . Magnetization measurements indicate the presence of ferromagnetic correlations with T{sub C}=55 K attributed to the exchange interactions for non-linear Co{sup 2+}-O-Sb{sup 5+}-O-Co{sup 2+} paths. The effective magnetic moment obtained experimentally is {mu}{sub exp}=4.38 {mu}{sub B} (per mol Co{sup 2+}), between the theoretical one for spin only (3.87 {mu}{sub B}) and spin-orbit value (6.63 {mu}{sub B}), indicating partially unquenched contribution. The low magnetization value at high magnetic field and low temperature (1 {mu}{sub B}/f.u., 5 T and 5 K) and the difference between ZFC and FC magnetization curves (at 5 kOe) indicate that the ferromagnetism do not reach a long range order and that the material has an important magnetic frustration. - Graphical abstract: Co-O-Co (Yellow octahedra only) rich zones (antiferromagnetic) are in contact with Co-O-Sb-O-Co (Red and yellow octahedra) rich zones (Ferromagnetic) to give the peculiar magnetic properties, as a consequence, a complex hysteresis loop can be observed composed by a main and irreversible curve in all the measured range, superimposed with a ferromagnetic component at low fields. Highlights: Black-Right-Pointing-Pointer La{sub 3}Co{sub 2}SbO{sub 9} has small Goldschmidt Tolerance Factor (t) due to the small size of La{sup 3+}. Black-Right-Pointing-Pointer Small t determines an angle for the path Co{sup 2+}-O-Sb{sup 5+}-O-Co{sup 2+} of 153 Degree-Sign . Black
International Nuclear Information System (INIS)
Franco, D.G.; Fuertes, V.C.; Blanco, M.C.; Fernández-Díaz, M.T.; Sánchez, R.D.; Carbonio, R.E.
2012-01-01
The synthesis, structural characterization, and magnetic properties of La 3 Co 2 SbO 9 double perovskite are reported. The crystal structure has been refined by X-ray and neutron powder diffraction data in the monoclinic space group P2 1 /n. Co 2+ and Sb 5+ have the maximum order allowed for the La 3 Co 2 SbO 9 stoichiometry. Rietveld refinements of powder neutron diffraction data show that at room temperature the cell parameters are a=5.6274(2) Å, b=5.6842(2) Å, c=7.9748(2) Å and β=89.999(3)°. Magnetization measurements indicate the presence of ferromagnetic correlations with T C =55 K attributed to the exchange interactions for non-linear Co 2+ –O–Sb 5+ –O–Co 2+ paths. The effective magnetic moment obtained experimentally is μ exp =4.38 μ B (per mol Co 2+ ), between the theoretical one for spin only (3.87 μ B ) and spin-orbit value (6.63 μ B ), indicating partially unquenched contribution. The low magnetization value at high magnetic field and low temperature (1 μ B /f.u., 5 T and 5 K) and the difference between ZFC and FC magnetization curves (at 5 kOe) indicate that the ferromagnetism do not reach a long range order and that the material has an important magnetic frustration. - Graphical abstract: Co–O–Co (Yellow octahedra only) rich zones (antiferromagnetic) are in contact with Co–O–Sb–O–Co (Red and yellow octahedra) rich zones (Ferromagnetic) to give the peculiar magnetic properties, as a consequence, a complex hysteresis loop can be observed composed by a main and irreversible curve in all the measured range, superimposed with a ferromagnetic component at low fields. Highlights: ► La 3 Co 2 SbO 9 has small Goldschmidt Tolerance Factor (t) due to the small size of La 3+ . ► Small t determines an angle for the path Co 2+ –O–Sb 5+ –O–Co 2+ of 153°. ► Ferromagnetism is attributed to exchange interactions for Co 2+ –O–Sb 5+ –O–Co 2+ paths. ► Ferromagnetic nanoclusters are embedded in an antiferromagnetic
Brown, P J; Neumann, K U; Smith, J G; Ziebeck, K R A
1997-01-01
The antiferromagnetic structure of the intermetallic compound U sub 1 sub 4 Au sub 5 sub 1 has been determined from neutron polarimetric measurements and refined by combining these data with integrated intensity measurements. The structure was found to be non-collinear with the U moments confined to the a-b plane. The moments of U atoms in each of the two sets of sixfold sites are arranged hexagonally with rotations of 60 deg. between them and the two sets are rotated with respect to one another by 50 deg. The third (twofold) set of U atoms has no ordered moment. These conclusions are in disagreement with a previous determination of the structure from powder data which gave a collinear structure with moments parallel to the c axis. Magnetization measurements made on single crystals in the temperature range 300-2 K can be understood in terms of a transition to a non-collinear easy plane antiferromagnetic structure stable below 22 K. Polarized neutron measurements have been used to determine the contribution of...
Energy Technology Data Exchange (ETDEWEB)
Sakhratov, Yu. A. [National High Magnetic Field Laboratory (United States); Svistov, L. E., E-mail: svistov@kapitza.ras.ru [Russian Academy Sciences, Kapitza Institute for Physical Problems (Russian Federation); Kuhns, P. L.; Zhou, H. D.; Reyes, A. P. [National High Magnetic Field Laboratory (United States)
2014-11-15
We have carried out {sup 63,65}Cu NMR spectra measurements in a magnetic field up to about 15.5 T on a single crystal of the multiferroic triangular-lattice antiferromagnet CuCrO{sub 2}. The measurements were performed for perpendicular and parallel orientations of the magnetic field with respect to the c axis of the crystal, and the detailed angle dependence of the spectra on the magnetic field direction in the ab plane was studied. The shape of the spectra can be well described in the model of spiral spin structure proposed by recent neutron diffraction experiments. When the field is rotated perpendicular to the crystal c axis, we observed, directly for the first time, a remarkable reorientation of the spin plane simultaneous with rotation of the incommensurate wavevector, by quantitatively deducing the conversion of the energetically less favorable domain to a more favorable one. At high enough fields parallel to the c axis, the data are consistent with either a field-induced commensurate spiral magnetic structure or an incommensurate spiral magnetic structure with a disorder in the c direction, suggesting that high fields may have influence on interplanar ordering.
Energy Technology Data Exchange (ETDEWEB)
Masrour, R., E-mail: rachidmasrour@hotmail.com [Laboratory of Materials, Processes, Environment and Quality, Cady Ayyed University, National School of Applied Sciences, BP. 63, 46000 Safi (Morocco); LMPHE (URAC 12), Faculty of Science, Mohammed V-Agdal University, Rabat (Morocco); Hlil, E.K. [Institut Néel, CNRS et Université Joseph Fourier, BP 166, F-38042 Grenoble Cedex 9 (France); Hamedoun, M. [Institute of Nanomaterials and Nanotechnologies, MAScIR, Rabat (Morocco); Benyoussef, A. [LMPHE (URAC 12), Faculty of Science, Mohammed V-Agdal University, Rabat (Morocco); Institute of Nanomaterials and Nanotechnologies, MAScIR, Rabat (Morocco); Hassan II Academy of Science and Technology, Rabat (Morocco); Mounkachi, O.; El Moussaoui, H. [Institute of Nanomaterials and Nanotechnologies, MAScIR, Rabat (Morocco)
2014-06-01
Self-consistent ab initio calculations, based on DFT (Density Functional Theory) approach and using FLAPW (Full potential Linear Augmented Plane Wave) method, are performed to investigate both electronic and magnetic properties of the MnSe lattice. Polarized spin and spin–orbit coupling are included in calculations within the framework of the antiferromagnetic state between two adjacent Mn lattices. Magnetic moments considered to lie along (001) axes are computed. Obtained data from ab initio calculations are used as input for the high temperature series expansions (HTSEs) calculations to compute other magnetic parameters. The zero-field high temperature static susceptibility series of the spin −4.28 nearest-neighbor Ising model on face centered cubic (fcc) and lattices is thoroughly analyzed by means of a power series coherent anomaly method (CAM). The exchange interaction between the magnetic atoms and the Néel temperature are deduced using the mean filed and HTSEs theories. - Highlights: • Ab initio calculations are used to investigate both electronic and magnetic properties of the MnSe alloys. • Obtained data from ab initio calculations are used as input for the HTSEs. • The Néel temperature is obtained for MnSe alloys.
Energy Technology Data Exchange (ETDEWEB)
Mizrahi, M., E-mail: mizrahi@fisica.unlp.edu.ar, E-mail: cabrera@fisica.unlp.edu.ar [INIFTA-CCT- La Plata-CONICET and Departamento de Física, Facultad de Ciencias Exactas, C. C. 67, Universidad Nacional de La Plata, 1900 La Plata (Argentina); Cabrera, A. F., E-mail: mizrahi@fisica.unlp.edu.ar, E-mail: cabrera@fisica.unlp.edu.ar; Desimoni, J. [IFLP-CCT-La Plata-CONICET and Departamento de Física, Facultad de Ciencias Exactas C.C. 67, Universidad Nacional de La Plata, 1900 La Plata (Argentina); Stewart, S. J. [IFLP-CCT-La Plata-CONICET and Departamento de Física, Facultad de Ciencias Exactas C.C. 67, Universidad Nacional de La Plata, 1900 La Plata (Argentina); Instituto Ciencias de la Salud, Universidad Nacional Arturo Jauretche, Av. Calchaquí No. 6200, Florencio Varela (Argentina)
2014-06-07
We report a magnetic study on nanostructured (Fe{sub 79}Mn{sub 21}){sub 1−x}Cu{sub x} (0.00 ≤ x ≤ 0.30) alloys using static magnetic measurements. The alloys are mainly composed by an antiferromagnetic fcc phase and a disordered region that displays a spin-glass-like behavior. The interplay between the antiferromagnetic and magnetically disordered phases establishes an exchange anisotropy that gives rise to a loop shift at temperatures below the freezing temperature of moments belonging to the disordered region. The loop shift is more noticeable as the Cu content increases, which also enhances the spin-glass-like features. Further, in the x = 0.30 alloy the alignment imposed by applied magnetic fields higher than 4 kOe prevail over the configuration determined by the frustration mechanism that characterizes the spin glass-like phase.
Nori, F.; Merlin, R.; Haas, S.; Sandvick, A.; Dagotto, E.
1996-03-01
We calculate(F. Nori, R.Merlin, S. Haas, A.W. Sandvik, and E. Dagotto, Physical Review Letters) 75, 553 (1995). the Raman spectrum of the two-dimensional (2D) spin-1/2 Heisenberg antiferromagnet by exact diagonalization and quantum Monte Carlo techniques on clusters of up to 144 sites. On a 16-site cluster, we consider the phonon-magnon interaction which leads to random fluctuations of the exchange integral. Results are in good agreement with experiments on various high-Tc precursors, such as La_2CuO4 and YBa_2Cu_3O_6.2. In particular, our calculations reproduce the broad lineshape of the two-magnon peak, the asymmetry about its maximum, the existence of spectral weight at high energies, and the observation of nominally forbidden A_1g scattering.
International Nuclear Information System (INIS)
Law, J M; Benner, H; Kremer, R K
2013-01-01
The temperature dependence of the spin susceptibilities of S = 1, 3/2 , 2, 5/2 and 7/2 Heisenberg antiferromagnetic 1D spins chains with nearest-neighbor coupling was simulated via quantum Monte Carlo calculations, within the reduced temperature range of 0.005 ≤ T* ≤ 100, and fitted to a Padé approximation with deviations between the simulated and fitted data of the same order of magnitude as or smaller than the quantum Monte Carlo simulation error. To demonstrate the practicality of our theoretical findings, we compare these results with the susceptibility of the well known 1D chain compound TMMC ([(CH 3 ) 4 N[MnCl 3
Energy Technology Data Exchange (ETDEWEB)
Zeng, Z.; Duan, Y.; Guenzburger, Diana [Centro Brasileiro de Pesquisas Fisicas (CBPF), Rio de Janeiro, RJ (Brazil)
1996-09-01
The electronic and magnetic properties of the nanometer-size antiferromagnet (the ferric wheel molecule) are investigated with the first-principles spin-polarized Discrete Variational Method, in the framework of Density Functional theory. Magnetic moments, densities of the states and charge and spin-density maps are obtained. The Moessbauer hyperfine parameters Isomer shift, Quadrupole Splitting and Hyperfine Field are obtained from the calculations and compared to reported experimental values when available. (author). 33 refs., 8 figs., 4 tabs.
Scattering of neutrons and critical phenomena in antiferromagnetic fermi liquid
International Nuclear Information System (INIS)
Akhiezer, I.A.; Barannik, E.A.
1980-01-01
The scattering of slow neutrons in an antiferromagnetic with collectivized magnetic electrons is considered and it is shown to significantly differ from the neutron scattering in an antiferromagnetic with localized magnetic electrons. The behaviour of scattering cross sections and fluctuation correlators near the Neel point is studied. These magnitudes are shown to increase with the critical index r=-1 [ru
International Nuclear Information System (INIS)
Gao, Bin; Weng, Yakui; Zhang, Jun-Jie; Zhang, Huimin; Zhang, Yang; Dong, Shuai
2017-01-01
Oxides with 4 d /5 d transition metal ions are physically interesting for their particular crystalline structures as well as the spin–orbit coupled electronic structures. Recent experiments revealed a series of 4 d /5 d transition metal oxides R 3 M O 7 (R : rare earth; M : 4 d /5 d transition metal) with unique quasi-one-dimensional M chains. Here first-principles calculations have been performed to study the electronic structures of La 3 OsO 7 and La 3 RuO 7 . Our study confirm both of them to be Mott insulating antiferromagnets with identical magnetic order. The reduced magnetic moments, which are much smaller than the expected value for ideal high-spin state (3 t 2g orbitals occupied), are attributed to the strong p − d hybridization with oxygen ions, instead of the spin–orbit coupling. The Ca-doping to La 3 OsO 7 and La 3 RuO 7 can not only modulate the nominal carrier density but also affect the orbital order as well as the local distortions. The Coulombic attraction and particular orbital order would prefer to form polarons, which might explain the puzzling insulating behavior of doped 5 d transition metal oxides. In addition, our calculations predict that the Ca-doping can trigger ferromagnetism in La 3 RuO 7 but not in La 3 OsO 7 . (paper)
Shape-induced anisotropy in antiferromagnetic nanoparticles
International Nuclear Information System (INIS)
Gomonay, O.; Kondovych, S.; Loktev, V.
2014-01-01
High fraction of the surface atoms considerably enhances the influence of size and shape on the magnetic and electronic properties of nanoparticles. Shape effects in ferromagnetic nanoparticles are well understood and allow us to set and control the parameters of a sample that affect its magnetic anisotropy during production. In the present paper we study the shape effects in the other widely used magnetic materials – antiferromagnets, – which possess vanishingly small or zero macroscopic magnetization. We take into account the difference between the surface and bulk magnetic anisotropy of a nanoparticle and show that the effective magnetic anisotropy depends on the particle shape and crystallographic orientation of its faces. The corresponding shape-induced contribution to the magnetic anisotropy energy is proportional to the particle volume, depends on magnetostriction, and can cause formation of equilibrium domain structure. Crystallographic orientation of the nanoparticle surface determines the type of domain structure. The proposed model allows us to predict the magnetic properties of antiferromagnetic nanoparticles depending on their shape and treatment. - Highlights: • We demonstrate that the shape effects in antiferromagnetic nanoparticles stem from the difference of surface and bulk magnetic properties combined with strong magnetoelastic coupling. • We predict shape-induced anisotropy in antiferromagnetic particles with large aspect ratio. • We predict different types of domain structures depending on the orientation of the particle faces
Antiferromagnetic resonance excited by oscillating electric currents
Sluka, Volker
2017-12-01
In antiferromagnetic materials the order parameter exhibits resonant modes at frequencies that can be in the terahertz range, making them interesting components for spintronic devices. Here, it is shown that antiferromagnetic resonance can be excited using the inverse spin-Hall effect in a system consisting of an antiferromagnetic insulator coupled to a normal-metal waveguide. The time-dependent interplay between spin torque, ac spin accumulation, and magnetic degrees of freedom is studied. It is found that the dynamics of the antiferromagnet affects the frequency-dependent conductivity of the normal metal. Further, a comparison is made between spin-current-induced and Oersted-field-induced excitation under the condition of constant power injection.
Energy Technology Data Exchange (ETDEWEB)
Batuk, Dmitry, E-mail: Dmitry.batuk@ua.ac.be [Electron Microscopy for Materials Research (EMAT), University of Antwerp, Groenenborgerlaan 171, B-2020, Antwerp (Belgium); De Dobbelaere, Christopher [Inorganic and Physical Chemistry Group, Hasselt University, Institute for Materials Research, Agoralaan Building D, B-3590, Diepenbeek (Belgium); Tsirlin, Alexander A. [National Institute of Chemical Physics and Biophysics, 12618, Tallinn (Estonia); Abakumov, Artem M. [Electron Microscopy for Materials Research (EMAT), University of Antwerp, Groenenborgerlaan 171, B-2020, Antwerp (Belgium); Hardy, An; Van Bael, Marlies K. [Inorganic and Physical Chemistry Group, Hasselt University, Institute for Materials Research, Agoralaan Building D, B-3590, Diepenbeek (Belgium); IMEC vzw, Division IMOMEC, Agoralaan Building D, B-3590, Diepenbeek (Belgium); Greenblatt, Martha [Department of Chemistry and Chemical Biology, Rutgers, State University of New Jersey, 610 Taylor Road, Piscataway, New Jersey, 08854-8087 (United States); Hadermann, Joke [Electron Microscopy for Materials Research (EMAT), University of Antwerp, Groenenborgerlaan 171, B-2020, Antwerp (Belgium)
2013-09-01
Graphical abstract: - Highlights: • The substitution of Cr for Mn in BiMnFe{sub 2}O{sub 6} is possible by the solution–gel method. • The BiCr{sub x}Mn{sub 1−x}Fe{sub 2}O{sub 6} solid solution is obtained for the x values up to 0.3. • Increasing Cr content lowers the temperature of the antiferromagnetic ordering. - Abstract: We report the Cr{sup 3+} for Mn{sup 3+} substitution in the BiMnFe{sub 2}O{sub 6} structure. The BiCr{sub x}Mn{sub 1−x}Fe{sub 2}O{sub 6} solid solution is obtained by the solution–gel synthesis technique for the x values up to 0.3. The crystal structure investigation using a combination of X-ray powder diffraction and transmission electron microscopy demonstrates that the compounds retain the parent BiMnFe{sub 2}O{sub 6} structure (for x = 0.3, a = 5.02010(6)Å, b = 7.06594(7)Å, c = 12.6174(1)Å, S.G. Pbcm, R{sub I} = 0.036, R{sub P} = 0.011) with only a slight decrease in the cell parameters associated with the Cr{sup 3+} for Mn{sup 3+} substitution. Magnetic susceptibility measurements suggest strong similarities in the magnetic behavior of BiCr{sub x}Mn{sub 1−x}Fe{sub 2}O{sub 6} (x = 0.2; 0.3) and parent BiMnFe{sub 2}O{sub 6}. Only T{sub N} slightly decreases upon Cr doping that indicates a very subtle influence of Cr{sup 3+} cations on the magnetic properties at the available substitution rates.
Spin Structure Analyses of Antiferromagnets
International Nuclear Information System (INIS)
Chung, Jae Ho; Song, Young Sang; Lee, Hak Bong
2010-05-01
We have synthesized series of powder sample of incommensurate antiferromagnetic multiferroics, (Mn, Co)WO 4 and Al doped Ba 0.5 Sr 1.5 Zn 2 Fe 12 O 22 , incommensurate antiferromagnetic multiferroics. Their spin structure was studied by using the HRPD. In addition, we have synthesized series of crystalline samples of incommensurate multiferroics, (Mn, Co)WO 4 and olivines. Their spin structure was investigated using neutron diffraction under high magnetic field. As a result, we were able to draw the phase diagram of (Mn, Co)WO 4 as a function of composition and temperature. We learned the how the spin structure changes with increased ionic substitution. Finally we have drawn the phase diagram of the multicritical olivine Mn2SiS4/Mn2GeS4 as a function of filed and temperature through the spin structure studies
Matsuda, K; Kohara, T; Amitsuka, H; Kuwahara, K; Matsumoto, T
2003-01-01
We have investigated the low-temperature phase appearing below T sub o = 17.5 K in URu sub 2 Si sub 2 by means of sup 2 sup 9 Si nuclear magnetic resonance (NMR) in a pressure range from 0 to 17.5 kbar across the pressure-induced phase transition at P sub c = 15 kbar. At pressures below P sub c , we have observed the sup 2 sup 9 Si NMR lines arising from antiferromagnetic (AF) and paramagnetic (PM) regions in the sample, giving evidence for a phase-separated AF ordering below T sub o. The AF region increases in volume fraction with increasing pressure up to P sub c. In the PM region, the temperature-dependence of the nuclear spin-lattice relaxation rate at Si sites shows a rapid decrease below T sub o , strongly suggesting the occurrence of a phase transition driven by a hidden order parameter. As applied pressure exceeds P sub c , the AF ordering appears uniformly at T sub o throughout the sample. In the pressure range from 0 to 17.5 kbar, the magnitude of the internal field at Si sites in the AF region rema...
DEFF Research Database (Denmark)
Mortensen, Kell; Tomkiewicz, Yaffa; Bechgaard, Klaus
1982-01-01
The anisotropy in the static magnetic susceptibility of bis-tetramethyltetraselenafulvalene hexafluoroarsenate [(TMTSF)2AsF6] has been investigated above and below the metal-to-insulator transition for a range of fields between 0.5 and 30 kG. The results are consistent with the expectations of a ...
Voltage Control of Antiferromagnetic Phases at Near-Terahertz Frequencies
Barra, Anthony; Domann, John; Kim, Ki Wook; Carman, Greg
2018-03-01
A method to control antiferromagnetism using voltage-induced strain is proposed and theoretically examined. Voltage-induced magnetoelastic anisotropy is shown to provide sufficient torque to switch an antiferromagnetic domain 90° either from out of plane to in plane or between in-plane axes. Numerical results indicate that strain-mediated antiferromagnetic switching can occur in an 80-nm nanopatterned disk at frequencies approaching 1 THz but that the switching speed heavily depends on the system's mechanical design. Furthermore, the energy cost to induce magnetic switching is only 450 aJ, indicating that magnetoelastic control of antiferromagnetism is substantially more energy efficient than other approaches.
Tunable Noncollinear Antiferromagnetic Resistive Memory through Oxide Superlattice Design
Hoffman, Jason D.; Wu, Stephen M.; Kirby, Brian J.; Bhattacharya, Anand
2018-04-01
Antiferromagnets (AFMs) have recently gathered a large amount of attention as a potential replacement for ferromagnets (FMs) in spintronic devices due to their lack of stray magnetic fields, invisibility to external magnetic probes, and faster magnetization dynamics. Their development into a practical technology, however, has been hampered by the small number of materials where the antiferromagnetic state can be both controlled and read out. We show that by relaxing the strict criterion on pure antiferromagnetism, we can engineer an alternative class of magnetic materials that overcome these limitations. This is accomplished by stabilizing a noncollinear magnetic phase in LaNiO3 /La2 /3Sr1 /3MnO3 superlattices. This state can be continuously tuned between AFM and FM coupling through varying the superlattice spacing, strain, applied magnetic field, or temperature. By using this alternative "knob" to tune magnetic ordering, we take a nanoscale materials-by-design approach to engineering ferromagneticlike controllability into antiferromagnetic synthetic magnetic structures. This approach can be used to trade-off between the favorable and unfavorable properties of FMs and AFMs when designing realistic resistive antiferromagnetic memories. We demonstrate a memory device in one such superlattice, where the magnetic state of the noncollinear antiferromagnet is reversibly switched between different orientations using a small magnetic field and read out in real time with anisotropic magnetoresistance measurements.
Spin transport and spin torque in antiferromagnetic devices
Železný, J.; Wadley, P.; Olejník, K.; Hoffmann, A.; Ohno, H.
2018-03-01
Ferromagnets are key materials for sensing and memory applications. In contrast, antiferromagnets, which represent the more common form of magnetically ordered materials, have found less practical application beyond their use for establishing reference magnetic orientations via exchange bias. This might change in the future due to the recent progress in materials research and discoveries of antiferromagnetic spintronic phenomena suitable for device applications. Experimental demonstration of the electrical switching and detection of the Néel order open a route towards memory devices based on antiferromagnets. Apart from the radiation and magnetic-field hardness, memory cells fabricated from antiferromagnets can be inherently multilevel, which could be used for neuromorphic computing. Switching speeds attainable in antiferromagnets far exceed those of ferromagnetic and semiconductor memory technologies. Here, we review the recent progress in electronic spin-transport and spin-torque phenomena in antiferromagnets that are dominantly of the relativistic quantum-mechanical origin. We discuss their utility in pure antiferromagnetic or hybrid ferromagnetic/antiferromagnetic memory devices.
Spin Transport in Ferromagnetic and Antiferromagnetic Textures
Akosa, Collins A.
2016-12-07
In this dissertation, we provide an accurate description of spin transport in magnetic textures and in particular, we investigate in detail, the nature of spin torque and magnetic damping in such systems. Indeed, as will be further discussed in this thesis, the current-driven velocity of magnetic textures is related to the ratio between the so-called non-adiabatic torque and magnetic damping. Uncovering the physics underlying these phenomena can lead to the optimal design of magnetic systems with improved efficiency. We identified three interesting classes of systems which have attracted enormous research interest (i) Magnetic textures in systems with broken inversion symmetry: We investigate the nature of magnetic damping in non-centrosymmetric ferromagnets. Based on phenomenological and microscopic derivations, we show that the magnetic damping becomes chiral, i.e. depends on the chirality of the magnetic texture. (ii) Ferromagnetic domain walls, skyrmions and vortices: We address the physics of spin transport in sharp disordered magnetic domain walls and vortex cores. We demonstrate that upon spin-independent scattering, the non-adiabatic torque can be significantly enhanced. Such an enhancement is large for vortex cores compared to transverse domain walls. We also show that the topological spin currents owing in these structures dramatically enhances the non-adiabaticity, an effect unique to non-trivial topological textures (iii) Antiferromagnetic skyrmions: We extend this study to antiferromagnetic skyrmions and show that such an enhanced topological torque also exist in these systems. Even more interestingly, while such a non-adiabatic torque inuences the undesirable transverse velocity of ferromagnetic skyrmions, in antiferromagnetic skyrmions, the topological non-adiabatic torque directly determines the longitudinal velocity. As a consequence, scaling down the antiferromagnetic skyrmion results in a much more efficient spin torque.
The electronic structure of antiferromagnetic chromium
DEFF Research Database (Denmark)
Skriver, Hans Lomholt
1981-01-01
The author has used the local spin density formalism to perform self-consistent calculations of the electronic structure of chromium in the non-magnetic and commensurate antiferromagnetic phases, as a function of the lattice parameter. A change of a few per cent in the atomic radius brings...
Theoretical modeling of diluted antiferromagnetic systems
International Nuclear Information System (INIS)
Pozo, J; Elgueta, R; Acevedo, R
2000-01-01
Some magnetic properties of a Diluted Antiferromagnetic System (DAFS) are studied. The model of the two sub-networks for antiferromagnetism is used and a Heisenberg Hamiltonian type is proposed, where the square operators are expressed in terms of boson operators with the approach of spin waves. The behavior of the diluted system's fundamental state depends basically on the competition effect between the anisotropy field and the Weiss molecular field. The approach used allows the diluted system to be worked for strong anisotropies as well as when these are very weak
Reciprocal propagation of surface modes in an antiferromagnetic film
International Nuclear Information System (INIS)
Oliveira, F.A.; Amato, M.A.
1987-09-01
Linear response theory is used to evaluate the Green's functions describing the fluctuations in an antiferromagnetic film at zero applied field. It is shown the similarities between the dielectric and magnetic excitations. (Author) [pt
Weyl magnons in breathing pyrochlore antiferromagnets
Li, Fei-Ye; Li, Yao-Dong; Kim, Yong Baek; Balents, Leon; Yu, Yue; Chen, Gang
2016-01-01
Frustrated quantum magnets not only provide exotic ground states and unusual magnetic structures, but also support unconventional excitations in many cases. Using a physically relevant spin model for a breathing pyrochlore lattice, we discuss the presence of topological linear band crossings of magnons in antiferromagnets. These are the analogues of Weyl fermions in electronic systems, which we dub Weyl magnons. The bulk Weyl magnon implies the presence of chiral magnon surface states forming arcs at finite energy. We argue that such antiferromagnets present a unique example, in which Weyl points can be manipulated in situ in the laboratory by applied fields. We discuss their appearance specifically in the breathing pyrochlore lattice, and give some general discussion of conditions to find Weyl magnons, and how they may be probed experimentally. Our work may inspire a re-examination of the magnetic excitations in many magnetically ordered systems. PMID:27650053
Role of structural factors in formation of chiral magnetic soliton lattice in Cr{sub 1/3}NbS₂
Energy Technology Data Exchange (ETDEWEB)
Volkova, L. M.; Marinin, D. V. [Institute of Chemistry, Far Eastern Branch of the Russian Academy of Sciences, 690022 Vladivostok (Russian Federation)
2014-10-07
The sign and strength of magnetic interactions not only between nearest neighbors, but also for longer-range neighbors in the Cr{sub 1/3}NbS₂ intercalation compound have been calculated on the basis of structural data. It has been found that left-handed spin helices in Cr{sub 1/3}NbS₂ are formed from strength-dominant at low temperatures antiferromagnetic (AFM) interactions between triangular planes of Cr³⁺ ions through the plane of just one of two crystallographically equivalent diagonals of side faces of embedded into each other trigonal prisms building up the crystal lattice of magnetic Cr³⁺ ions. These helices are oriented along the c axis and packed into two-dimensional triangular lattices in planes perpendicular to these helices directions and lay one upon each other with a displacement. The competition of the above AFM helices with weaker inter-helix AFM interactions could promote the emergence of a long-period helical spin structure. One can assume that in this case, the role of Dzyaloshinskii-Moriya interaction consists of final ordering and stabilization of chiral spin helices into a chiral magnetic soliton lattice. The possibility of emergence of solitons in M{sub 1/3}NbX{sub 2} and M{sub 1/3}TaX₂ (M = Cr, V, Ti, Rh, Ni, Co, Fe, and Mn; X = S and Se) intercalate compounds has been examined. Two important factors caused by the crystal structure (predominant chiral magnetic helices and their competition with weaker inter-helix interactions not destructing the system quasi-one-dimensional character) can be used for the crystal chemistry search of solitons.
Heat-driven spin torques in antiferromagnets
Białek, Marcin; Bréchet, Sylvain; Ansermet, Jean-Philippe
2018-04-01
Heat-driven magnetization damping, which is a linear function of a temperature gradient, is predicted in antiferromagnets by considering the sublattice dynamics subjected to a heat-driven spin torque. This points to the possibility of achieving spin torque oscillator behavior. The model is based on the magnetic Seebeck effect acting on sublattices which are exchange coupled. The heat-driven spin torque is estimated and the feasibility of detecting this effect is discussed.
Quantum ballistic transport by interacting two-electron states in quasi-one-dimensional channels
Energy Technology Data Exchange (ETDEWEB)
Huang, Danhong [Air Force Research Laboratory, Space Vehicles Directorate, Kirtland Air Force Base, New Mexico 87117 (United States); Center for High Technology Materials, University of New Mexico, 1313 Goddard St SE, Albuquerque, New Mexico 87106 (United States); Gumbs, Godfrey [Center for High Technology Materials, University of New Mexico, 1313 Goddard St SE, Albuquerque, New Mexico 87106 (United States); Abranyos, Yonatan [Department of Physics and Astronomy, Hunter College of the City University of New York, 695 Park Avenue, New York, New York 10065 (United States); Pepper, Michael; Kumar, Sanjeev [Department of Electronic and Electrical Engineering, University College London, London, WC1E 7JE (United Kingdom); London Centre for Nanotechnology, 17-19 Gordon Street, London, WC1H 0AH (United Kingdom)
2015-11-15
For quantum ballistic transport of electrons through a short conduction channel, the role of Coulomb interaction may significantly modify the energy levels of two-electron states at low temperatures as the channel becomes wide. In this regime, the Coulomb effect on the two-electron states is calculated and found to lead to four split energy levels, including two anticrossing-level and two crossing-level states. Moreover, due to the interplay of anticrossing and crossing effects, our calculations reveal that the ground two-electron state will switch from one anticrossing state (strong confinement) to a crossing state (intermediate confinement) as the channel width gradually increases and then back to the original anticrossing state (weak confinement) as the channel width becomes larger than a threshold value. This switching behavior leaves a footprint in the ballistic conductance as well as in the diffusion thermoelectric power of electrons. Such a switching is related to the triple spin degeneracy as well as to the Coulomb repulsion in the central region of the channel, which separates two electrons away and pushes them to different channel edges. The conductance reoccurrence region expands from the weak to the intermediate confinement regime with increasing electron density.
Revealing origin of quasi-one dimensional current transport in defect rich two dimensional materials
DEFF Research Database (Denmark)
Lotz, Mikkel Rønne; Boll, Mads; Hansen, Ole
2014-01-01
to a non-uniform current flow characteristic of lower dimensionality. In this work, simulations based on a finite element method together with a Monte Carlo approach are used to establish the transition from 2D to quasi-1D current transport, when applying a micro four-point probe to measure on 2D...... conductors with an increasing amount of line-shaped defects. Clear 2D and 1D signatures are observed at low and high defect densities, respectively, and current density plots reveal the presence of current channels or branches in defect configurations yielding 1D current transport. A strong correlation...
DEFF Research Database (Denmark)
Sing, M.; Schwingenschlögl, U.; Claessen, R.
2003-01-01
We have thoroughly characterized the surfaces of the organic charge-transfer salts TTF-TCNQ and (TMTSF)(2)PF6 which are generally acknowledged as prototypical examples of one-dimensional conductors. In particular x-ray-induced photoemission spectroscopy turns out to be a valuable nondestructive...
International Nuclear Information System (INIS)
Nguyen Minh Khue; Solyom, J.
1980-03-01
The novel method proposed by one of the authors to calculate exactly the response functions of the one-dimensional Tomonaga-model is described in more detail. The method is generalized for the case of a system of coupled chains where both the interchain and interchain interactions have forward scattering components only. The model does not show real phase transition at any finite temperature indicating that the interchain backward scattering or hopping is needed to have an ordering of the chains at finite temperature. (author)
International Nuclear Information System (INIS)
Cuevas, J.; Malomed, Boris A.; Kevrekidis, P. G.; Frantzeskakis, D. J.
2009-01-01
We study families of one-dimensional matter-wave bright solitons supported by the competition of contact and dipole-dipole (DD) interactions of opposite signs. Soliton families are found, and their stability is investigated in the free space and in the presence of an optical lattice (OL). Free-space solitons may exist with an arbitrarily weak local attraction if the strength of the DD repulsion is fixed. In the case of the DD attraction, solitons do not exist beyond a maximum value of the local-repulsion strength. In the system which includes the OL, a stability region for subfundamental solitons is found in the second finite band gap. For the existence of gap solitons (GSs) under the attractive DD interaction, the contact repulsion must be strong enough. In the opposite case of the DD repulsion, GSs exist if the contact attraction is not too strong. Collisions between solitons in the free space are studied too. In the case of the local attraction, they merge or pass through each other at small and large velocities, respectively. In the presence of the local repulsion, slowly moving solitons bounce from each other.
Strongly correlated quasi-one-dimensional bands: Ground states, optical absorption, and phonons
International Nuclear Information System (INIS)
Campbell, D.K.; Gammel, J.T.; Loh, E.Y. Jr.
1989-01-01
Using the Lanczos method for exact diagonalization on systems up to 14 sites, combined with a novel ''phase randomization'' technique for extracting more information from these small systems, we investigate several aspects of the one-dimensional Peierls-Hubbard Hamiltonian, in the context of trans-polyacetylene: the dependence of the ground state dimerization on the strength of the electron-electron interactions, including the effects of ''off-diagonal'' Coulomb terms generally ignored in the Hubbard model; the phonon vibrational frequencies and dispersion relations, and the optical absorption properties, including the spectrum of absorptions as a function of photon energy. These three different observables provide considerable insight into the effects of electron-electron interactions on the properties of real materials and thus into the nature of strongly correlated electron systems. 29 refs., 11 figs
Sidewall gated double well quasi-one-dimensional resonant tunneling transistors
Kolagunta, V. R.; Janes, D. B.; Melloch, M. R.; Youtsey, C.
1997-12-01
We present gating characteristics of submicron vertical resonant tunneling transistors in double quantum well heterostructures. Current-voltage characteristics at room temperature and 77 K for devices with minimum feature widths of 0.9 and 0.7 μm are presented and discussed. The evolution of the I-V characteristics with increasing negative gate biases is related to the change in the lateral confinement, with a transition from a large area 2D to a quasi-1D. Even gating of multiple wells and lateral confinement effects observable at 77 K make these devices ideally suited for applications in multi-valued logic systems and low-dimensional structures.
Lagrangian Particle Tracking Simulation for Warm-Rain Processes in Quasi-One-Dimensional Domain
Kunishima, Y.; Onishi, R.
2017-12-01
Conventional cloud simulations are based on the Euler method and compute each microphysics process in a stochastic way assuming infinite numbers of particles within each numerical grid. They therefore cannot provide the Lagrangian statistics of individual particles in cloud microphysics (i.e., aerosol particles, cloud particles, and rain drops) nor discuss the statistical fluctuations due to finite number of particles. We here simulate the entire precipitation process of warm-rain, with tracking individual particles. We use the Lagrangian Cloud Simulator (LCS), which is based on the Euler-Lagrangian framework. In that framework, flow motion and scalar transportation are computed with the Euler method, and particle motion with the Lagrangian one. The LCS tracks particle motions and collision events individually with considering the hydrodynamic interaction between approaching particles with a superposition method, that is, it can directly represent the collisional growth of cloud particles. It is essential for trustworthy collision detection to take account of the hydrodynamic interaction. In this study, we newly developed a stochastic model based on the Twomey cloud condensation nuclei (CCN) activation for the Lagrangian tracking simulation and integrated it into the LCS. Coupling with the Euler computation for water vapour and temperature fields, the initiation and condensational growth of water droplets were computed in the Lagrangian way. We applied the integrated LCS for a kinematic simulation of warm-rain processes in a vertically-elongated domain of, at largest, 0.03×0.03×3000 (m3) with horizontal periodicity. Aerosol particles with a realistic number density, 5×107 (m3), were evenly distributed over the domain at the initial state. Prescribed updraft at the early stage initiated development of a precipitating cloud. We have confirmed that the obtained bulk statistics fairly agree with those from a conventional spectral-bin scheme for a vertical column domain. The centre of the discussion will be the Lagrangian statistics which is collected from the individual behaviour of the tracked particles.
Backscattering from width variations in quasi-one-dimensional strips of topological insulators
International Nuclear Information System (INIS)
Takagaki, Y
2012-01-01
Conductance modulations in wide-narrow-wide electron waveguides constructed from a two-dimensional topological insulator are investigated numerically. The conductance exhibits the Fabry-Perot oscillation at the opening of the helical edge states in the narrow segment when the potential offset imposed in the segment is varied. The quantum multiple reflections between the two ends of the narrow segment manifested by the oscillation demonstrate that the topological states are not protected from the scattering caused by an abrupt change in the channel width. The bulk states do not affect the vulnerability against the geometry scattering but they give rise to resonant transmission in an unconventional fashion.
Dark and bright solitons in a quasi-one-dimensional Bose-Einstein condensate
International Nuclear Information System (INIS)
Wang, Shun-Jin; Jia, Cheng-Long; An, Jun-Hong; Zhao, Dun; Luo, Hong-Gang
2003-01-01
The analytical dark and bright soliton solutions of the one-dimensional Gross-Pitaevskii equation with a confining potential are obtained. For the bright soliton, the recent experimental finding is studied, and the particle number of the soliton and the window of the particle numbers for the bright soliton to occur are estimated analytically and in good agreement with the experimental data. The existence of dark soliton for the attractive interaction and bright soliton for the repulsive interaction is predicted under proper conditions
Revealing origin of quasi-one dimensional current transport in defect rich two dimensional materials
International Nuclear Information System (INIS)
Lotz, Mikkel R.; Boll, Mads; Bøggild, Peter; Petersen, Dirch H.; Hansen, Ole; Kjær, Daniel
2014-01-01
The presence of defects in graphene have for a long time been recognized as a bottleneck for its utilization in electronic and mechanical devices. We recently showed that micro four-point probes may be used to evaluate if a graphene film is truly 2D or if defects in proximity of the probe will lead to a non-uniform current flow characteristic of lower dimensionality. In this work, simulations based on a finite element method together with a Monte Carlo approach are used to establish the transition from 2D to quasi-1D current transport, when applying a micro four-point probe to measure on 2D conductors with an increasing amount of line-shaped defects. Clear 2D and 1D signatures are observed at low and high defect densities, respectively, and current density plots reveal the presence of current channels or branches in defect configurations yielding 1D current transport. A strong correlation is found between the density filling factor and the simulation yield, the fraction of cases with 1D transport and the mean sheet conductance. The upper transition limit is shown to agree with the percolation threshold for sticks. Finally, the conductance of a square sample evaluated with macroscopic edge contacts is compared to the micro four-point probe conductance measurements and we find that the micro four-point probe tends to measure a slightly higher conductance in samples containing defects
Proton conductivity in quasi-one dimensional hydrogen-bonded systems: A nonlinear approach
International Nuclear Information System (INIS)
Tsironis, G.; Phevmatikos, S.
1988-01-01
Defect formation and transport in a hydrogen-bonded system is studied via a two-sublattice soliton-bearing one-dimensional model. Ionic and orientational defects are associated with distinct nonlinear topological excitations in the present model. The dynamics of these excitations is studied both analytically and with the use of numerical simulations. It is shown that the two types of defects are soliton solutions of a double Sine--Gordon equation which describes the motion of the protons in the long-wavelength limit. With each defect there is an associated deformation in the ionic lattice that, for small speeds, follows the defect dynamically albeit resisting its motion. Free propagation as well as collision properties of the proton solitons are presented. 33 refs., 10 figs
Du, Xiang
As the sizes of individual components in electronic and optoelectronic devices approach nano scale, the performance of the devices is often determined by surface properties due to their large surface-to-volume ratio. Surface phenomena have become one of the cornerstones in nanoelectronic industry. For this reason, research on the surface functionalization has been tremendous amount of growth over the past decades, and promises to be an increasingly important field in the future. Surface functionalization, as an effective technique to modify the surface properties of a material through a physical or chemical approach, exhibits great potential to solve the problems and challenges, and modulate the performance of nanomaterials based functional devices. Surface functionalization drives the developments and applications of modern electronic and optoelectronic devices fabricated by nanomaterials. In this thesis, I demonstrate two surface functionalization approaches, namely, surface transfer doping and H2 annealing, to effectively solve the problems and significantly enhance the performance of 2D (single structure black phosphorus (BP) and heterostructure graphene/Si Schottky junction), and quasi-1D (molybdenum trioxide (MoO 3) nanobelt) nanomaterials based functional devices, respectively. In situ photoelectron spectroscopy (PES) measurements were also carried out to explore the interfacial charge transfer occurring at the interface between the nanostructures and doping layers, and the gap states in MoO 3 thin films, which provides the underlying mechanism to understand and support our device measurement results. In the first part of this thesis, I will discuss the first surface functionalization approach, namely, surface transfer doping, to effectively modulate the ambipolar characteristics of 2D few-layer BP flakes based FETs. The ambipolar characteristics of BP transistors were effectively modulated through in situ surface functionalization with cesium carbonate (Cs2CO3) and MoO3, respectively. Cs2CO3 was found to strongly electron dope black phosphorus. The electron mobility of black phosphorus was significantly enhanced to ˜27 cm2V-1s-1 after 10 nm Cs2CO3 modification, indicating a greatly improved electron transport behavior. In contrast, MoO3 decoration demonstrated a giant hole doping effect. In situ PES characterization confirms the interfacial charge transfer between black phosphorus and doping layers. This doping can also modulate the Schottky junctions formed between metal contacts and black phosphorus flakes, and hence to enhance the responsivity of black phosphorus based photodetectors. These findings coupled with the tunable nature of the surface transfer doping scheme ensure black phosphorus as a promising candidate for further complementary logic electronics. Following the same surface transfer doping technique, I will demonstrate a remarkable performance enhancement of graphene/Si Schottky junction based self-powered photodetectors via surface modification with MoO3 thin film. It was found that the photocurrent responsivity of MoO3 doped graphene/Si photodetectors was highly increased under a wide spectrum of illuminated light from ultraviolet to near infrared. The current on-off ratio reached up to ˜104 under illumination of 500 nm light with intensity of ˜62 muWcm-2. More importantly, the external quantum efficiency of graphene/Si devices was significantly enhanced up to ˜80% by almost four times in the visible light region after MoO3 functionalization. The largely improved photodetecting performance originates from the increased Schottky barrier height at the graphene/Si interface as well as the reduced series resistance after MoO3 modification, which was further corroborated by the in situ PES and electrical transport characterizations. These observations promise a simple method to effectively modify the graphene/Si Schottky junction based self-powered photodetectors and thus significantly enhance their photodetecting performance. After discussion of the first surface functionalization method, next I will introduce the second approach which is H2 annealing, to greatly extend the photoresponse range of single MoO3 nanobelt based photodetector from UV to visible light by introducing substantial gap states. After annealing, the conductance of MoO3 nanobelt was largely enhanced; at the same time, the photodetector possessed wide visible spectrum response. As corroborated by in situ PES investigations, such strong wide spectrum photoresponse arises from the largely enriched oxygen vacancies and gap states in MoO3 nanobelt after H2 annealing. These results open up a new avenue to extend the wide bandgap metal oxide nanomaterials based optoelectronics devices with efficient visible light response through surface modification, i.e. the introduction of the high density of carefully engineered gap states.
Faraday waves in quasi-one-dimensional superfluid Fermi-Bose mixtures
DEFF Research Database (Denmark)
Abdullaev, F. Kh.; Ögren, Magnus; Sørensen, Mads Peter
2013-01-01
The generation of Faraday waves in superfluid Fermi-Bose mixtures in elongated traps is investigated. The generation of waves is achieved by periodically changing a parameter of the system in time. Two types of modulations of parameters are considered: a variation of the fermion-boson scattering...... length and the boson-boson scattering length. We predict the properties of the generated Faraday patterns and study the parameter regions where they can be excited....
Pankrats, A I; Demidov, A A; Ritter, C; Velikanov, D A; Semenov, S V; Tugarinov, V I; Temerov, V L; Gudim, I A
2016-10-05
The magnetic structure of the mixed rare-earth system Pr x Y1-x Fe3(BO3)4 (x = 0.75, 0.67, 0.55, 0.45, 0.25) was studied via magnetic and resonance measurements. These data evidence the successive spin reorientation from the easy-axis antiferromagnetic structure formed in PrFe3(BO3)4 to the easy-plane one of YFe3(BO3)4 associated with the weakening of the magnetic anisotropy of the Pr subsystem due to its diamagnetic dilution by nonmagnetic Y. This reorientation occurs through the formation of an inclined magnetic structure, as was confirmed by our previous neutron research in the range of x = 0.67 ÷ 0.45. In the compounds with x = 0.75 and 0.67 whose magnetic structure is close to the easy-axis one, a two-step spin reorientation takes place in the magnetic field H||c. Such a peculiarity is explained by the formation of an interjacent inclined magnetic structure with magnetic moments of Fe ions located closer to the basal plane than in the initial state, with these intermediate states remaining stable in some ranges of the magnetic field. An approach based on a crystal field model for the Pr(3+) ion and the molecular-field approximation is used to describe the magnetic characteristics of the system Pr x Y1-x Fe3(BO3)4. With the parameters of the d-d and f-d exchange interactions, of the magnetic anisotropy of the iron subsystem and of the crystal field parameters of praseodymium thus determined, it is possible to achieve a good agreement between the experimental and calculated temperature and field dependences of the magnetization curves (up to 90 kOe) and magnetic susceptibilities (2-300 K).
Enhanced antiferromagnetic coupling in dual-synthetic antiferromagnet with Co2FeAl electrodes
International Nuclear Information System (INIS)
Zhang, D.L.; Xu, X.G.; Wu, Y.; Li, X.Q.; Miao, J.; Jiang, Y.
2012-01-01
We study dual-synthetic antiferromagnets (DSyAFs) using Co 2 FeAl (CFA) Heusler electrodes with a stack structure of Ta/CFA/Ru/CFA/Ru/CFA/Ta. When the thicknesses of the two Ru layers are 0.45 nm, 0.65 nm or 0.45 nm, 1.00 nm, the CFA-based DSyAF has a strong antiferromagnetic coupling between adjacent CFA layers at room temperature with a saturation magnetic field of ∼11,000 Oe, a saturation magnetization of ∼710 emu/cm 3 and a coercivity of ∼2.0 Oe. Moreover, the DSyAF has a good thermal stability up to 400 °C, at which CFA films show B2-ordered structure. Therefore, the CFA-based DSyAFs are favorable for applications in future spintronic devices. - Graphical abstract: Display Omitted Highlights: ► Co 2 FeAl can be applied in room temperature dual-synthetic antiferromagnets. ► Co 2 FeAl dual-synthetic antiferromagnets have a good thermal stability up to 400 °C. ► The Co 2 FeAl has B2-ordered structure in annealed dual-synthetic antiferromagnets.
Energy Technology Data Exchange (ETDEWEB)
Glaria, Arnaud [CNRS, LCC (Laboratoire de Chimie de Coordination), 205, route de Narbonne, F-31077 Toulouse (France); Universite de Toulouse, UPS, INPT, LCC, F-31077 Toulouse (France); Kahn, Myrtil L., E-mail: myrtil.kahn@lcc-toulouse.fr [CNRS, LCC (Laboratoire de Chimie de Coordination), 205, route de Narbonne, F-31077 Toulouse (France); Universite de Toulouse, UPS, INPT, LCC, F-31077 Toulouse (France); Chaudret, Bruno [CNRS, LCC (Laboratoire de Chimie de Coordination), 205, route de Narbonne, F-31077 Toulouse (France); Universite de Toulouse, UPS, INPT, LCC, F-31077 Toulouse (France); Lecante, Pierre; Casanove, Marie-Jose [CNRS, CEMES (Centre d' Elaboration des Materiaux et d' Etudes Structurales), 29 rue Jeanne Marvig, BP 4347, 31055 Toulouse Cedex (France); Barbara, Bernard, E-mail: bernard.barbara@grenoble.cnrs.fr [Institut Louis Neel, CNRS, 25 Av. des martyrs, BP 166, 38042 Grenoble Cedex 09 (France)
2011-09-15
Highlights: {yields} Pure Wuestite (Fe{sub 1-y}O) nanoparticles synthesized by organometallic chemistry. {yields} The influence of the surface ligands on the magnetic properties. {yields} Ferromagnetic core-antiferromagnetic shell magnetic nanoparticles. - Abstract: Wuestite particles (Fe{sub 1-y}O) are synthesized using controlled hydrolysis at room temperature of [Fe(N(SiMe{sub 3}){sub 2}){sub 2}] and stabilized by amine ligands. This method leads to 5 nm pure wuestite particles. This phase is clearly identified by transmission electron microscopy and wide angle X-ray scattering. Distortion in the crystallographic structure has been demonstrated. Particular attention is paid on the Fe(III) formation. Moreover, a combination of Moessbauer spectroscopy and SQuID measurements, revealed that the particles are composed of an antiferromagnetic core surrounded by a ferromagnetic shell. According to the Neel theory, the Fe(III) and Fe(II) ions present in the particles are ferromagnetically coupled and the proportion of Fe(III) ions varies from 3.9 to 7.1% as a function of the amine ligand.
Antiferromagnetic spin-orbitronics
Manchon, Aurelien; Saidaoui, Hamed Ben Mohamed; Ghosh, Sumit
2015-01-01
Antiferromagnets have long remained an intriguing and exotic state of matter, whose application has been restricted to enabling interfacial exchange bias in metallic and tunneling spin-valves [1]. Their role in the expanding field of applied spintronics has been mostly passive and the in-depth investigation of their basic properties mostly considered from a fundamental perspective.
Nanoparticles of antiferromagnetic materials
DEFF Research Database (Denmark)
Madsen, Daniel Esmarch
2008-01-01
I denne Ph.D. afhandling studeres forskellige egenskaber ved antiferromagnetiske nanopartikler. I en ideel antiferromagnet er spinnene orienteret således at der ikke er et resulterende magnetisk moment. I nanopartikler af antiferromagnetiske materialer er denne kompensation på grund af forskellig...
Antiferromagnetic spin-orbitronics
Manchon, Aurelien
2015-05-01
Antiferromagnets have long remained an intriguing and exotic state of matter, whose application has been restricted to enabling interfacial exchange bias in metallic and tunneling spin-valves [1]. Their role in the expanding field of applied spintronics has been mostly passive and the in-depth investigation of their basic properties mostly considered from a fundamental perspective.
Long-range interactions in antiferromagnetic quantum spin chains
Bravo, B.; Cabra, D. C.; Gómez Albarracín, F. A.; Rossini, G. L.
2017-08-01
We study the role of long-range dipolar interactions on antiferromagnetic spin chains, from the classical S →∞ limit to the deep quantum case S =1 /2 , including a transverse magnetic field. To this end, we combine different techniques such as classical energy minima, classical Monte Carlo, linear spin waves, bosonization, and density matrix renormalization group (DMRG). We find a phase transition from the already reported dipolar ferromagnetic region to an antiferromagnetic region for high enough antiferromagnetic exchange. Thermal and quantum fluctuations destabilize the classical order before reaching magnetic saturation in both phases, and also close to zero field in the antiferromagnetic phase. In the extreme quantum limit S =1 /2 , extensive DMRG computations show that the main phases remain present with transition lines to saturation significatively shifted to lower fields, in agreement with the bosonization analysis. The overall picture maintains a close analogy with the phase diagram of the anisotropic XXZ spin chain in a transverse field.
Energy Technology Data Exchange (ETDEWEB)
Gao, R.L. [School of Metallurgy and Materials Engineering, Chongqing University of Science and Technology, Chongqing 401331 (China); Xu, Z.Y., E-mail: zhyxu@nim.ac.cn [National Institute of Metrology, Beijing 100029 (China); Wang, L.C. [State Key Laboratory for Magnetism, Institute of Physics, Chinese Academy of Sciences, Beijing 100190 (China); Dong, Q.Y.; Zhang, Y. [Department of Physics, Capital Normal University, Beijing 100048 (China); Liu, F.H. [National Space Science Center, Beijing 100190 (China); Mo, Z.J. [School of material Science and Engineering, Hebei University of Technology, Tianjin 300401 (China); Niu, E. [State Key Laboratory for Magnetism, Institute of Physics, Chinese Academy of Sciences, Beijing 100190 (China); Fu, C.L.; Cai, W.; Chen, G.; Deng, X.L. [School of Metallurgy and Materials Engineering, Chongqing University of Science and Technology, Chongqing 401331 (China)
2015-05-15
Highlights: • Antiferromagnetic material RCu{sub x}Ge{sub 2} of high purity was prepared. • Large MCE as −10.2 J/kg K and −10.5 J/kg K for RCu{sub x}Ge{sub 2} (Ho, Er) was obtained for field change of 0–50 kOe. • The RCu{sub x}Ge{sub 2} compounds with variable x had different transition temperature which made them suitable for ‘table-like’ magnetocaloric refrigerant. - Abstract: Magnetic properties and magnetocaloric effect (MCE) of HoCu{sub 0.33}Ge{sub 2} and ErCu{sub 0.25}Ge{sub 2} compounds have been investigated. The compounds were determined to be antiferromagnetic with the Néel temperatures T{sub N} = 9 K and 3.9 K, respectively. The critical transition magnetic fields for the metamagnetic transition from antiferromagnetic to ferromagnetic state below T{sub N} were determined to be 10 kOe for HoCu{sub 0.33}Ge{sub 2} at 5 K and 6 kOe for ErCu{sub 0.25}Ge{sub 2} at 2 K. Large MCE with the maximal values of magnetic entropy changes (ΔS{sub M}) as −10.2 J/kg K at 10.5 K were found in HoCu{sub 0.33}Ge{sub 2} for field changes of 0–70 kOe and −10.5 J/kg K at 5.5 K in ErCu{sub 0.25}Ge{sub 2} for field changes of 0–50 kOe, respectively. The large ΔS{sub M} around T{sub N} as well as no hysteresis loss made RCu{sub x}Ge{sub 2} competitive candidates as low temperature magnetic refrigerant.
Antiferromagnetic transition in graphene functionalized with nitroaniline
Komlev, Anton A.; Makarova, Tatiana L.; Lahderanta, Erkki; Semenikhin, Petr Valeryevich; Veinger, Anatoly I.; Kochman, Igor V.; Magnani, Giacomo; Bertoni, Giovanni; Pontiroli, Daniele; Ricco, Mauro
2017-07-01
Magnetic properties of graphene nanostructures functionalized with aromatic radicals were investigated by electron spin resonance (ESR) and superconducting quantum interference device (SQUID) techniques. Three types of functionalized graphene samples were investigated (functionalization was performed by 4-bromoaniline, 4-nitroaniline, or 4-chloroaniline). According to SQUID measurements, in case of functionalization by nitroaniline, sharp change in temperature dependence of magnetic susceptibility was observed near 120 K. Such behavior was explained as antiferromagnetic ordering. The same but more extended effect was observed in ESR measurements below 160 K. In the ESR measurements, only one resonance line with g-factor equal to 2.003 was observed. Based on the temperature dependencies of spin concentration and resonance position and intensity, the effect was explained as antiferromagnetic ordering along the extended defects on the basal planes of the graphene.
Electronic energy spectra in antiferromagnetic media with broken reciprocity
International Nuclear Information System (INIS)
Vitebsky, I.; Edelkind, J.; Bogachek, E.N.; Scherbakov, A.G.; Landman, U.
1997-01-01
Electronic energy spectra var-epsilon(q) of antiferromagnetically ordered media may display nonreciprocity; that is, the energies corresponding to Bloch states with wave numbers q and -q may be different. In this paper a simple Kronig-Penney model, which includes a staggered microscopic magnetic and electric fields of the proper symmetry, is employed to estimate the magnitude of nonreciprocity effects in systems such as antiferromagnetically ordered crystals as well as periodical layered structures. copyright 1997 The American Physical Society
Reversal of exchange bias in nanocrystalline antiferromagnetic-ferromagnetic bilayers
International Nuclear Information System (INIS)
Prados, C; Pina, E; Hernando, A; Montone, A
2002-01-01
The sign of the exchange bias in field cooled nanocrystalline antiferromagnetic-ferromagnetic bilayers (Co-O and Ni-O/permalloy) is reversed at temperatures approaching the antiferromagnetic (AFM) blocking temperature. A similar phenomenon is observed after magnetic training processes at similar temperatures. These effects can be explained assuming that the boundaries of nanocrystalline grains in AFM layers exhibit lower transition temperatures than grain cores
Energy Technology Data Exchange (ETDEWEB)
Plumier, R [Commissariat a l' Energie Atomique, Saclay (France). Centre d' Etudes Nucleaires
1969-07-01
Magnetic structure determination of a few ferri- and antiferromagnets normal spinels has led us to study what are, besides nearest neighbour magnetic interactions, the magnetic terms which have to be considered in the establishment of such or such magnetic structure. Tetragonal distortion which is frequently observed in such compounds is of the order of magnetic exchange striction (10{sup -3}). Such a distortion leads to two effects. First it decreases the total energy of the system. Secondly it introduces term of axial magnetic anisotropy. Besides this term of axial anisotropy, the possibility of basal anisotropy in the case of coplanar magnetic structure has to be considered. This last term explained why the magnetic structures of such antiferromagnetic spinels frequently have one or more cell parameters which are twice that of the chemical cell. Finally the comparison between various magnetic structures of antiferromagnetic spinels in which the leading term is the magnetic energy between first nearest neighbours, shows that the part played by magnetic interactions between non nearest neighbours is not negligible. Such indirect superexchange interactions through two anions or two anions and a cation on tetrahedral site, although of the order of a few percent of the preceding one, join a given ion to its twelve second nearest neighbours, six third nearest neighbours and twelve fourth nearest neighbours. (author) [French] La determination des structures magnetiques de quelques spinelles ferri- et antiferromagnetiques normaux nous a conduit a preciser quels sont, en dehors du terme dominant d'interaction magnetique entre ions premiers voiins, les termes d'energie magnetique a considerer dans l'apparition de telle ou telle structure magnetique. La distorsion quadratique que l'on observe frequemment dans ces composes est de l'ordre de grandeur de celle attribuable a la striction d'echange (10{sup -3}). L'effet d'une telle distorsion est double. Non seulement elle
Noncollinear antiferromagnetic Mn3Sn films
Markou, A.; Taylor, J. M.; Kalache, A.; Werner, P.; Parkin, S. S. P.; Felser, C.
2018-05-01
Noncollinear hexagonal antiferromagnets with almost zero net magnetization were recently shown to demonstrate giant anomalous Hall effect. Here, we present the structural and magnetic properties of noncollinear antiferromagnetic Mn3Sn thin films heteroepitaxially grown on Y:ZrO2 (111) substrates with a Ru underlayer. The Mn3Sn films were crystallized in the hexagonal D 019 structure with c -axis preferred (0001) crystal orientation. The Mn3Sn films are discontinuous, forming large islands of approximately 400 nm in width, but are chemical homogeneous and characterized by near perfect heteroepitaxy. Furthermore, the thin films show weak ferromagnetism with an in-plane uncompensated magnetization of M =34 kA/m and coercivity of μ0Hc=4.0 mT at room temperature. Additionally, the exchange bias effect was studied in Mn3Sn /Py bilayers. Exchange bias fields up to μ0HEB=12.6 mT can be achieved at 5 K. These results show Mn3Sn films to be an attractive material for applications in antiferromagnetic spintronics.
Antiferromagnetic phase of the gapless semiconductor V3Al
Jamer, M. E.; Assaf, B. A.; Sterbinsky, G. E.; Arena, D.; Lewis, L. H.; Saúl, A. A.; Radtke, G.; Heiman, D.
2015-03-01
Discovering new antiferromagnetic (AF) compounds is at the forefront of developing future spintronic devices without fringing magnetic fields. The AF gapless semiconducting D 03 phase of V3Al was successfully synthesized via arc-melting and annealing. The AF properties were established through synchrotron measurements of the atom-specific magnetic moments, where the magnetic dichroism reveals large and oppositely oriented moments on individual V atoms. Density functional theory calculations confirmed the stability of a type G antiferromagnetism involving only two-thirds of the V atoms, while the remaining V atoms are nonmagnetic. Magnetization, x-ray diffraction, and transport measurements also support the antiferromagnetism. This archetypal gapless semiconductor may be considered as a cornerstone for future spintronic devices containing AF elements.
International Nuclear Information System (INIS)
Vidal, J.-P.; Vidal-Valat, G.; Kurki-Suonio, K.
2004-01-01
X-ray diffraction intensities from CoO were measured above and below the Neel temperature. The data were submitted to a non-parametric multipole analysis aiming at formulation of experimentally valid statements on the nature of the charge distribution. Strong 'bonding maxima' are seen between the Co O nearest neighbors. In the paramagnetic state they are formed by the Co-ion alone, in the antiferromagnetic state they involve a strong CoO coupling. The outer electrons of oxygen give rise to slight maxima in the directions, making the atom into an O 2- ion. In the paramagnetic state, their coupling with the bonding feature forms an octahedral electron cage around each oxygen atom. Broad density maxima between the atoms in directions are present in both states. They connect the 'bonding maxima' in the directions, more strongly in the antiferromagnetic state, building up an interatomic three-dimensional network. Such electron network structures seem to be characteristic of metal oxides more generally
Magnetic reconnection and current sheet formation in 3D magnetic configurations
International Nuclear Information System (INIS)
Frank, A.G.
1999-01-01
The problem of magnetic reconnection in three-dimensional (3D) magnetic configurations has been studied experimentally. The research has concentrated on the possibilities of formation of current sheets, which represent crucial objects for a realization of magnetic reconnection phenomena. Different types of 3D magnetic configurations were examined, including configurations with singular lines of the X-type, non-uniform fields containing isolated magnetic null-points and without null-points. It was revealed that formation of quasi-one-dimensional current sheets is the universal process for plasma dynamics in 3D magnetic fields both with null-points and without. At the same time the peculiarities of current sheets, plasma dynamics and magnetic reconnection processes depend essentially on characteristics of 3D magnetic configurations. The result of principal significance obtained was that magnetic reconnection phenomena can take place in a wide range of 3D magnetic configurations as a consequence of their ability to form current sheets. (author)
Magnetoresistive properties of non-uniform state of antiferromagnetic semiconductors
International Nuclear Information System (INIS)
Krivoruchko, V.N.
1996-01-01
The phenomenological model of magnetoresistive properties of magneto-non-single-phase state of alloyed magnetic semiconductors is considered using the concept derived for a description of magnetoresistive effects in layered and granular magnetic metals. By assuming that there exists a magneto-non-single state in the manganites having the perovskite structure, it is possible to describe, in the framework of above approach, large magnetoresistive effects of manganite phases with antiferromagnetic order and semiconductor-type conductivity as well as those with antiferromagnetic properties and metallic-type conductivity
Isothermal anisotropic magnetoresistance in antiferromagnetic metallic IrMn.
Galceran, R; Fina, I; Cisneros-Fernández, J; Bozzo, B; Frontera, C; López-Mir, L; Deniz, H; Park, K-W; Park, B-G; Balcells, Ll; Martí, X; Jungwirth, T; Martínez, B
2016-10-20
Antiferromagnetic spintronics is an emerging field; antiferromagnets can improve the functionalities of ferromagnets with higher response times, and having the information shielded against external magnetic field. Moreover, a large list of aniferromagnetic semiconductors and metals with Néel temperatures above room temperature exists. In the present manuscript, we persevere in the quest for the limits of how large can anisotropic magnetoresistance be in antiferromagnetic materials with very large spin-orbit coupling. We selected IrMn as a prime example of first-class moment (Mn) and spin-orbit (Ir) combination. Isothermal magnetotransport measurements in an antiferromagnetic-metal(IrMn)/ferromagnetic-insulator thin film bilayer have been performed. The metal/insulator structure with magnetic coupling between both layers allows the measurement of the modulation of the transport properties exclusively in the antiferromagnetic layer. Anisotropic magnetoresistance as large as 0.15% has been found, which is much larger than that for a bare IrMn layer. Interestingly, it has been observed that anisotropic magnetoresistance is strongly influenced by the field cooling conditions, signaling the dependence of the found response on the formation of domains at the magnetic ordering temperature.
Mn2Au: Body-centered-tetragonal bimetallic antiferromagnets grown by molecular beam epitataxy
Czech Academy of Sciences Publication Activity Database
Wu, H.C.; Liao, Z.M.; Sofin, R.G.S.; Feng, G.; Ma, X.M.; Shick, Alexander; Mryasov, O. N.; Shvets, I.V.
2012-01-01
Roč. 24, č. 47 (2012), s. 6374-6379 ISSN 0935-9648 Institutional research plan: CEZ:AV0Z10100520 Keywords : antiferromagnets * antiferromagnetic spintronics * exchange bias * molecular beam epitaxy Subject RIV: BM - Solid Matter Physics ; Magnetism Impact factor: 14.829, year: 2012
Long range order in the ground state of two-dimensional antiferromagnets
International Nuclear Information System (INIS)
Neves, E.J.; Perez, J.F.
1985-01-01
The existence of long range order is shown in the ground state of the two-dimensional isotropic Heisenberg antiferromagnet for S >= 3/2. The method yields also long range order for the ground state of a larger class of anisotropic quantum antiferromagnetic spin systems with or without transverse magnetic fields. (Author) [pt
Effect of low transverse magnetic field on the confinement strength in a quasi-1D wire
International Nuclear Information System (INIS)
Kumar, Sanjeev; Thomas, K. J.; Smith, L. W.; Farrer, I.; Ritchie, D. A.; Jones, G. A. C.; Griffiths, J.; Pepper, M.
2013-01-01
Transport measurements in a quasi-one dimensional (1D) quantum wire are reported in the presence of low transverse magnetic field. Differential conductance shows weak quantised plateaus when the 2D electrons are squeezed electrostatically. Application of a small transverse magnetic field (0.2T) enhances the overall degree of quantisation due to the formation of magneto-electric subbands. The results show the role of magnetic field to fine tune the confinement strength in low density wires when interaction gives rise to double row formation
Anisotropic magnetoresistance in an antiferromagnetic semiconductor
Czech Academy of Sciences Publication Activity Database
Fina, I.; Martí, Xavier; Yi, D.; Liu, J.; Chu, J.-H.; Rayan-Serrao, C.; Suresha, S.; Shick, Alexander; Železný, Jakub; Jungwirth, Tomáš; Fontcuberta, J.; Ramesh, R.
2014-01-01
Roč. 5, SEP (2014), "4671-1"-"4671-7" ISSN 2041-1723 R&D Projects: GA MŠk(CZ) LM2011026; GA ČR GB14-37427G; GA ČR(CZ) GAP204/10/0330 EU Projects: European Commission(XE) 268066 - 0MSPIN Grant - others:AV ČR(CZ) AP0801 Program:Akademická prémie - Praemium Academiae Institutional support: RVO:68378271 Keywords : antiferromagnets * semiconductors * spintronics Subject RIV: BM - Solid Matter Physics ; Magnetism Impact factor: 11.470, year: 2014
Room-temperature antiferromagnetic memory resistor
Czech Academy of Sciences Publication Activity Database
Martí, Xavier; Fina, I.; Frontera, C.; Liu, J.; Wadley, P.; He, P.; Paull, R.J.; Clarkson, J.D.; Kudrnovský, Josef; Turek, Ilja; Kuneš, Jan; Yi, D.; Chu, J.-H.; Nelson, C.T.; You, L.; Arenholz, E.; Salahuddin, S.; Fontcuberta, J.; Jungwirth, Tomáš; Ramesh, R.
2014-01-01
Roč. 13, č. 4 (2014), s. 367-374 ISSN 1476-1122 R&D Projects: GA MŠk(CZ) LM2011026; GA ČR(CZ) GAP204/11/1228 EU Projects: European Commission(XE) 268066 - 0MSPIN Grant - others:AV ČR(CZ) AP0801 Program:Akademická prémie - Praemium Academiae Institutional support: RVO:68378271 ; RVO:68081723 Keywords : spintronics * antiferromagnets * memories Subject RIV: BM - Solid Matter Physics ; Magnetism Impact factor: 36.503, year: 2014
Solitons in one-dimensional antiferromagnetic chains
International Nuclear Information System (INIS)
Pires, A.S.T.; Talim, S.L.; Costa, B.V.
1989-01-01
We study the quantum-statistical mechanics, at low temperatures, of a one-dimensional antiferromagnetic Heisenberg model with two anisotropies. In the weak-coupling limit we determine the temperature dependences of the soliton energy and the soliton density. We have found that the leading correction to the sine-Gordon (SG) expression for the soliton density and the quantum soliton energy comes from the out-of-plane magnon mode, not present in the pure SG model. We also show that when an external magnetic field is applied, the chain supports a new type of kink, where the sublattices rotate in opposite directions
Electric control of antiferromagnets
Czech Academy of Sciences Publication Activity Database
Fina, I.; Martí, Xavier
2017-01-01
Roč. 53, č. 2 (2017), 1-7, č. článku 2500107. ISSN 0018-9464 R&D Projects: GA ČR GB14-37427G EU Projects: European Commission(XE) 268066 - 0MSPIN Institutional support: RVO:68378271 Keywords : magnetoelectric effects * perpendicular magnetic anisotropy * magnetic domain walls * magnetic domains * switches * magnetic fields Subject RIV: BM - Solid Matter Physics ; Magnetism OBOR OECD: Condensed matter physics (including formerly solid state physics, supercond.) Impact factor: 1.243, year: 2016
Quantum Number Fractionalization in Antiferromagnets
Laughlin, R. B.; Giuliano, D.; Caracciolo, R.; White, O.
1998-01-01
This is a pedagogical introduction to the mathematics of 1-dimensional spin-1/2 antiferromagnets. Topics covered include the Haldane-Shastry Hamiltonian, vector ``supercharges'', conserved spin currents, spinons, the supersymmetric Kuramoto-Yokoyama Hamiltonian, and holons.
Excitations in a Two-Dimensional Random Antiferromagnet
DEFF Research Database (Denmark)
Birgeneau, R. J.; Walker, L. R.; Guggenheim, H. J.
1975-01-01
Inelastic neutron scattering studies of the magnetic excitations in the planar Heisenberg random antiferromagnet Rb2Mn0.5Ni0.5F4 at 7K are reported. Two well-defined bands of excitations are observed. A simple mean crystal model is found to predict accurately the measured dispersion relations using...
Antiferromagnetic ground state in NpCoGe
Czech Academy of Sciences Publication Activity Database
Colineau, E.; Griveau, J.C.; Eloirdi, R.; Gaczyński, P.; Khmelevskyi, S.; Shick, Alexander; Caciuffo, R.
2014-01-01
Roč. 89, č. 11 (2014), "115135-1"-"115135-11" ISSN 1098-0121 R&D Projects: GA ČR(CZ) GAP204/10/0330 Institutional support: RVO:68378271 Keywords : neptunium * anti-ferromagnetism * quantum critical phenomena Subject RIV: BM - Solid Matter Physics ; Magnetism Impact factor: 3.736, year: 2014
235U NMR study of the itinerant antiferromagnet USb2
International Nuclear Information System (INIS)
Kato, Harukazu; Sakai, Hironori; Ikushima, Kenji; Kambe, Shinsaku; Tokunaga, Yo; Aoki, Dai; Haga, Yoshinori; O-bar nuki, Yoshichika; Yasuoka, Hiroshi; Walstedt, Russell E.
2005-01-01
We have succeeded in resolving a 235 U antiferromagnetic nuclear magnetic resonance (AFNMR) signal using 235 U-enriched samples of USb 2 . The uranium hyperfine field and coupling constant estimated for this compound are consistent with those from other experiments. This is the first reported observation of 235 U NMR in conducting host material
NdRhSn: A ferromagnet with an antiferromagnetic precursor
Czech Academy of Sciences Publication Activity Database
Mihalik, M.; Prokleška, J.; Kamarád, Jiří; Prokeš, K.; Isnard, O.; McIntyre, G. J.; Dönni, A.; Yoshii, S.; Kitazawa, H.; Sechovský, V.; de Boer, F.R.
2011-01-01
Roč. 83, č. 10 (2011), "104403-1"-"104403-10" ISSN 1098-0121 R&D Projects: GA ČR GA202/09/1027 Institutional research plan: CEZ:AV0Z10100521 Keywords : NdRhSn * ferromagnet * antiferromagnetic precursor Subject RIV: BM - Solid Matter Physics ; Magnetism Impact factor: 3.691, year: 2011
Spin Hall magnetoresistance in antiferromagnet/normal metal bilayers
Manchon, Aurelien
2017-01-01
We investigate the emergence of spin Hall magnetoresistance in a magnetic bilayer composed of a normal metal adjacent to an antiferromagnet. Based on a recently derived drift diffusion equation, we show that the resistance of the bilayer depends on the relative angle between the direction transverse to the current flow and the Néel order parameter. While this effect presents striking similarities with the spin Hall magnetoresistance recently reported in ferromagnetic bilayers, its physical origin is attributed to the anisotropic spin relaxation of itinerant spins in the antiferromagnet.
ZnFe{sub 2}O{sub 4} antiferromagnetic structure redetermination
Energy Technology Data Exchange (ETDEWEB)
Kremenović, Aleksandar, E-mail: akremenovic@rgf.bg.ac.rs [Laboratory for Crystallography, Faculty of Mining and Geology, University of Belgrade, Đušina 7, Belgrade 11000 (Serbia); Antić, Bratislav [Condensed Matter Physics Laboratory, Institute of Nuclear Sciences “Vinča”, University of Belgrade, P.O. Box 522, Belgrade 11001 (Serbia); Vulić, Predrag [Laboratory for Crystallography, Faculty of Mining and Geology, University of Belgrade, Đušina 7, Belgrade 11000 (Serbia); Blanuša, Jovan [Condensed Matter Physics Laboratory, Institute of Nuclear Sciences “Vinča”, University of Belgrade, P.O. Box 522, Belgrade 11001 (Serbia); Tomic, Aleksandra [Condensed Matter Physics Laboratory, Institute of Nuclear Sciences “Vinča”, University of Belgrade, P.O. Box 522, Belgrade 11001 (Serbia); Department of Applied Physics and Applied Mathematics, Columbia University, New York, NY, 10027 (United States)
2017-03-15
Magnetic structure of ZnFe{sub 2}O{sub 4} normal spinel is re-examined. Antiferromagnetic structure non-collinear model is established within C{sub a}2 space group having four different crystallographic/magnetic sites for 32 Fe{sup 3+} spins within magnetic unit cell. - Highlights: • Magnetic structure of ZnFe{sub 2}O{sub 4} normal spinel is re-examined. • Antiferromagnetic non-collinear structure model is established within C{sub a}2 space group. • Four different crystallographic/magnetic sites contain 32 Fe{sup 3+} spins within magnetic unit cell.
Energy Technology Data Exchange (ETDEWEB)
Krebs, J [Commissariat a l' Energie Atomique, Saclay (France). Centre d' Etudes Nucleaires
1968-01-01
In this thesis we describe a pulsed field device with which we obtain magnetization curves up to 450 kOE at all temperatures between 1. 6 and 300. We have studied the 'spin-flopping'(and therefore the anisotropy) in MnF{sub 2} versus temperature, below the Neel point. We have also studied the antiferromagnets MnSO{sub 4}. and MnSO{sub 4}.H{sub 2}O which have revealed saturation fields respectively of 250 kOE and 320 kOE. (author) [French] Ce memoire est consacre a la fabrication et a la mise au point d'un appareillage utilisant la decharge d'une batterie de condensateurs, afin de faire des mesures d'aimantation en champs pulses jusqu'a 450 kOE a toute temperature entre 1,6 K et 300 K. Nous avons etudie le deplacement de la transition de 'spin-flopping' dans MnF{sub 2} en fonction de la temperature et nous en avons deduit la variation de la constante d'anisotropie en fonction de T au-dessous du point de Neel. Nous avons egalement fait l'etude magnetique des antiferromagnetiques MnSO{sub 4} et MnSO{sub 4}.H{sub 2}O et nous avons mis en evidence la saturation de ces deux substances pour des champs respectifs de 250 kOE et 320 kOE. (auteur)
Escuer, Albert; Vicente, Ramon; Kumar, Sujit B.; Solans, Xavier; Font-Bardía, Mercé; Caneschi, Andrea
1996-05-22
The trinuclear complex (&mgr;(3)-CO(3))[Ni(3)(Medpt)(3)(NCS)(4)] was obtained by reaction of basic solutions of nickel(II), Medpt (bis(3aminopropyl)methylamine) and thiocyanate ligand with atmospheric CO(2) or by simple reaction with carbonate anion. (&mgr;(3)-CO(3))[Ni(3)(Medpt)(3)(NCS)(4)] crystallizes in the triclinic system, space group P&onemacr;, with a = 12.107(5) Å, b = 12.535(7) Å, c = 16.169(9) Å, alpha = 102.69(5) degrees, beta = 92.91(5) degrees, gamma = 118.01(4) degrees, Z = 2, and R = 0.043. The three nickel atoms are asymmetrically bridged by one pentadentate carbonato ligand, which shows a novel coordination mode. The (&mgr;(3)-CO(3))[Ni(3)(Medpt)(3)(NCS)(4)] compound shows a very strong antiferromagnetic coupling. Fit as irregular triangular arrangement gave J(1) = -88.4, J(2) = -57.7, and J(3) = -9.6 cm(-)(1), which is the strongest AF coupling observed to date for Ni(3) compounds. The magnetic behavior of the carbonato bridge is discussed.
Lee, W.-J.; Do, S.-H.; Lee, S.; Choi, Y.-S.; Choi, K.-Y.; Yoon, Sungwon; Suh, Byoungjin; Jang, Zeehoon
2018-01-01
We report on the spin dynamics of the strong spin-orbit coupled antiferromagnets Ba3Ru1- x Ir x Ti2O9 ( x = 0.5 and 0.8), which comprise a mixture of edge- and corner-sharing triangles. Muon spin-relaxation measurements give no hints of long-range magnetic order down to 25 mK. Rather, the muon spin-relaxation rates λ( T) show persistent spin dynamics below 1 K, indicating that fast fluctuations are dominant in spite of Ir4+( J eff = 1/2)/Ru4+( S = 1) randomness. The muon spin depolarization of both compounds is well described by a stretched exponential function with the stretching exponent β = 0.4 (0.6) for x = 0.5 (0.8) at low temperatures, which is larger than β = 1/3 expected for a spin glass. Our results suggest that randomness in the spin number and the exchange interaction induces a partial spin freezing, but the majority of spins remain dynamically fluctuating.
A neutron scattering study on the antiferromagnet in an exchange biased systems
Energy Technology Data Exchange (ETDEWEB)
Solina, Danica; Lott, Dieter; Fenske, Jochen; Schreyer, Andreas [Institute of Materials Research, GKSS Research Centre, Geesthacht (Germany); Schmidt, Wolfgang [Institut-Laue-Langevin, Grenoble (France); Wu, Yu-Chang; Lai, Chih-Huang [Department of Materials Science and Engineering, National Tsing Hua University, HsinChu (China)
2008-07-01
The magnetic structure of single crystal antiferromagnetic PtMn that biases CoFe has been studied using neutron scattering. Polarized neutron reflection (PNR) was used to determine the switching behaviour of the ferromagnetic layer and polarized neutron diffraction (PND) to probe the magnetic configuration of the anti-ferromagnetic layer. PNR suggests a combination of rotation and domain formation. Changes were observed in the PND patterns taken at points around the hysteresis loop. The diffraction data has been simulated with a 'twisting' of part of the anti-ferromagnetic layer as the ferromagnetic layer changes.
Room-temperature antiferromagnetic memory resistor.
Marti, X; Fina, I; Frontera, C; Liu, Jian; Wadley, P; He, Q; Paull, R J; Clarkson, J D; Kudrnovský, J; Turek, I; Kuneš, J; Yi, D; Chu, J-H; Nelson, C T; You, L; Arenholz, E; Salahuddin, S; Fontcuberta, J; Jungwirth, T; Ramesh, R
2014-04-01
The bistability of ordered spin states in ferromagnets provides the basis for magnetic memory functionality. The latest generation of magnetic random access memories rely on an efficient approach in which magnetic fields are replaced by electrical means for writing and reading the information in ferromagnets. This concept may eventually reduce the sensitivity of ferromagnets to magnetic field perturbations to being a weakness for data retention and the ferromagnetic stray fields to an obstacle for high-density memory integration. Here we report a room-temperature bistable antiferromagnetic (AFM) memory that produces negligible stray fields and is insensitive to strong magnetic fields. We use a resistor made of a FeRh AFM, which orders ferromagnetically roughly 100 K above room temperature, and therefore allows us to set different collective directions for the Fe moments by applied magnetic field. On cooling to room temperature, AFM order sets in with the direction of the AFM moments predetermined by the field and moment direction in the high-temperature ferromagnetic state. For electrical reading, we use an AFM analogue of the anisotropic magnetoresistance. Our microscopic theory modelling confirms that this archetypical spintronic effect, discovered more than 150 years ago in ferromagnets, is also present in AFMs. Our work demonstrates the feasibility of fabricating room-temperature spintronic memories with AFMs, which in turn expands the base of available magnetic materials for devices with properties that cannot be achieved with ferromagnets.
New antiferromagnetic semiconductor CuCr1.5Sb0.5S4
International Nuclear Information System (INIS)
Kesler, Ya.A.; Koroleva, L.I.; Mikheev, M.G.; Odintsov, A.G.; Filimonov, D.S.
1993-01-01
New halcogenide compound with spinel-antiferromagnetic semiconductor CuCr 1.5 Sb 0.5 S 4 are obtained and studied for the first time. Magnetic properties of this compound, namely, magnetization linear dependence, maximum on PHI(T) curve in the low-temperature area and realization of the Curie-Weis law for paramagnetic susceptibility with negative paramagnetic temperature testiby to the fact that this compound is antiferromagnetic
Nuclear spin-magnon relaxation in two-dimensional Heisenberg antiferromagnets
International Nuclear Information System (INIS)
Wal, A.J. van der.
1979-01-01
Experiments are discussed of the dependence on temperature and magnetic field of the longitudinal relaxation time of single crystals of antiferromagnetically ordered insulators, i.e. in the temperature range below the Neel temperature and in fields up to the spin-flop transition. The experiments are done on 19 F nuclei in the Heisenberg antiferromagnets K 2 MnF 4 and K 2 NiF 4 , the magnetic structure of which is two-dimensional quadratic. (C.F.)
Identifying Two-Dimensional Z 2 Antiferromagnetic Topological Insulators
Bègue, F.; Pujol, P.; Ramazashvili, R.
2018-01-01
We revisit the question of whether a two-dimensional topological insulator may arise in a commensurate Néel antiferromagnet, where staggered magnetization breaks the symmetry with respect to both elementary translation and time reversal, but retains their product as a symmetry. In contrast to the so-called Z 2 topological insulators, an exhaustive characterization of antiferromagnetic topological phases with the help of topological invariants has been missing. We analyze a simple model of an antiferromagnetic topological insulator and chart its phase diagram, using a recently proposed criterion for centrosymmetric systems [13]. We then adapt two methods, originally designed for paramagnetic systems, and make antiferromagnetic topological phases manifest. The proposed methods apply far beyond the particular examples treated in this work, and admit straightforward generalization. We illustrate this by two examples of non-centrosymmetric systems, where no simple criteria have been known to identify topological phases. We also present, for some cases, an explicit construction of edge states in an antiferromagnetic topological insulator.
Polarized Neutron Reflectivity Simulation of Ferromagnet/ Antiferromagnet Thin Films
Energy Technology Data Exchange (ETDEWEB)
Kim, Ki Yeon; Lee, Jeong Soo
2008-02-15
This report investigates the current simulating and fitting programs capable of calculating the polarized neutron reflectivity of the exchange-biased ferromagnet/antiferromagnet magnetic thin films. The adequate programs are selected depending on whether nonspin flip and spin flip reflectivities of magnetic thin films and good user interface are available or not. The exchange-biased systems such as Fe/Cr, Co/CoO, CoFe/IrMn/Py thin films have been simulated successfully with selected programs.
Antiferromagnetism in reduced YBa2Cu3O6+x
International Nuclear Information System (INIS)
Casalta, H.; Schleger, P.; Montfrooij, W.; Andersen, N.H.; Lebech, B.; Liang Ruixing; Hardy, W.N.
1995-01-01
Magnetic ordering was investigated by neutron scattering in an YBa 2 Cu 3 O 6+x single crystal. We observed antiferromagnetic ordering (AFI) (T N =410 K for x=0.1 and T N =368 K for x=0.18), but found no evidence for a reordering down to 2 K (AFII). The magnetic structure factors are presented to emphasize the anisotropic character of the form factor. ((orig.))
Interface states in stressed semiconductor heterojunction with antiferromagnetic ordering
International Nuclear Information System (INIS)
Kantser, V.G.
1995-08-01
The stressed heterojunctions with antiferromagnetic ordering in which the constituents have opposite band edge symmetry and their gaps have opposite signs have been investigated. The interface states have been shown to appear in these heterojunctions and they are spin-split. As a result if the Fermi level gets into one of the interface bands then it leads to magnetic ordering in the interface plane. That is if the interface magnetization effect can be observed. (author). 14 refs, 2 figs
Antiferromagnetic spinor condensates in a bichromatic superlattice
Tang, Tao; Zhao, Lichao; Chen, Zihe; Liu, Yingmei
2017-04-01
A spinor Bose-Einstein condensate in an optical supelattice has been considered as a good quantum simulator for understanding mesoscopic magnetism. We report an experimental study on an antiferromagnetic spinor condensate in a bichromatic superlattice constructed by a cubic red-detuned optical lattice and a one-dimensional blue-detuned optical lattice. Our data demonstrate a few advantages of this bichromatic superlattice over a monochromatic lattice. One distinct advantage is that the bichromatic superlattice enables realizing the first-order superfluid to Mott-insulator phase transitions within a much wider range of magnetic fields. In addition, we discuss an apparent discrepancy between our data and the mean-field theory. We thank the National Science Foundation and the Oklahoma Center for the Advancement of Science and Technology for financial support.
Magnetostriction and magnetoelastic domains in antiferromagnets
International Nuclear Information System (INIS)
Gomonay, Helen; Loktev, Vadim M.
2002-01-01
The problem of the observable equilibrium domain structure (DS) in pure antiferromagnets is investigated with the use of continuous elasticity theory. It is shown that the difference between the bulk and surface magnetoelastic strains causes imaginary 'incompatibility elastic charges' analogous to the surface 'magnetic' charges in ferromagnets. The corresponding long-range field is shown to contribute to the 'stray' energy of the sample that governs the appearance of the DS, the contribution from the 'elastic charges' being proportional to the sample volume. Competition between the elastic 'stray' field, which favours inhomogeneous strain distribution, and an external field, which tends to make the sample homogeneous, provides a reversible reconstruction of the DS under the action of the external magnetic field. (author)
DEFF Research Database (Denmark)
Lindgård, P.-A.; Schmid, B.
1993-01-01
In the singlet ground-state systems CsFeCl3 and CsFeBr3 a large single-ion anisotropy causes a singlet ground state and a doubly degenerate doublet as the first excited states of the Fe2+ ion. In addition the magneteic interaction is anisotropic being much larger along the z axis than perpendicular...... to it. Therefore, these quasi-one-dimensional magnetic model systems are ideal to demonstrate unique correlation effects. Within the framework of the correlation theory we derive the expressions for the excitation spectrum. When a magnetic field is applied parallel to the z axis both substances have...
Polarized neutron powder diffraction studies of antiferromagnetic order in bulk and nanoparticle NiO
DEFF Research Database (Denmark)
Brok, Erik; Lefmann, Kim; Deen, Pascale P.
2015-01-01
surface contribution to the magnetic anisotropy. Here we explore the potential use of polarized neutron diffraction to reveal the magnetic structure in NiO bulk and nanoparticle powders by applying the XYZ-polarization analysis method. Our investigations address in particular the spin orientation in bulk....... The results show that polarization analyzed neutron powder diffraction is a viable method to investigate magnetic order in powders of antiferromagnetic nanoparticles.......In many materials it remains a challenge to reveal the nature of magnetic correlations, including antiferromagnetism and spin disorder. Revealing the spin structure in magnetic nanoparticles is further complicated by the large incoherent neutron scattering cross section from water adsorbed...
Spin transfer torque in antiferromagnetic spin valves: From clean to disordered regimes
Saidaoui, Hamed Ben Mohamed
2014-05-28
Current-driven spin torques in metallic spin valves composed of antiferromagnets are theoretically studied using the nonequilibrium Green\\'s function method implemented on a tight-binding model. We focus our attention on G-type and L-type antiferromagnets in both clean and disordered regimes. In such structures, spin torques can either rotate the magnetic order parameter coherently (coherent torque) or compete with the internal antiferromagnetic exchange (exchange torque). We show that, depending on the symmetry of the spin valve, the coherent and exchange torques can either be in the plane, ∝n×(q×n) or out of the plane ∝n×q, where q and n are the directions of the order parameter of the polarizer and the free antiferromagnetic layers, respectively. Although disorder conserves the symmetry of the torques, it strongly reduces the torque magnitude, pointing out the need for momentum conservation to ensure strong spin torque in antiferromagnetic spin valves.
Spin transfer torque in antiferromagnetic spin valves: From clean to disordered regimes
Saidaoui, Hamed Ben Mohamed; Manchon, Aurelien; Waintal, Xavier
2014-01-01
Current-driven spin torques in metallic spin valves composed of antiferromagnets are theoretically studied using the nonequilibrium Green's function method implemented on a tight-binding model. We focus our attention on G-type and L-type antiferromagnets in both clean and disordered regimes. In such structures, spin torques can either rotate the magnetic order parameter coherently (coherent torque) or compete with the internal antiferromagnetic exchange (exchange torque). We show that, depending on the symmetry of the spin valve, the coherent and exchange torques can either be in the plane, ∝n×(q×n) or out of the plane ∝n×q, where q and n are the directions of the order parameter of the polarizer and the free antiferromagnetic layers, respectively. Although disorder conserves the symmetry of the torques, it strongly reduces the torque magnitude, pointing out the need for momentum conservation to ensure strong spin torque in antiferromagnetic spin valves.
Magnetic field effect on the ground-state binding energy in InGaN/GaN parabolic QWW
International Nuclear Information System (INIS)
El Ghazi, Haddou; Jorio, Anouar; Zorkani, Izeddine
2013-01-01
Within the framework of the effective mass scheme, the ground-state binding energy of hydrogenic shallow-donor impurity in wurtzite (WZ) (In,Ga)N/GaN parabolic transversal-section quantum-well wire (PQWW) subjected to magnetic field is investigated. The finite-difference method within the quasi-one-dimensional effective potential model is used. A cylindrical QWW effective radius is introduced to describe the lateral confinement strength. The results show that: (i) the binding energy is the largest for the impurity located at a point corresponding to the largest electron probability density and (ii) it increases with increasing external magnetic field
Magnetic field effect on the ground-state binding energy in InGaN/GaN parabolic QWW
Energy Technology Data Exchange (ETDEWEB)
El Ghazi, Haddou, E-mail: hadghazi@gmail.com [LPS, Faculty of sciences, Dhar EL Mehrez, B.P 1796 Atlas Fez (Morocco); Specials Mathematics, CPGE Kénitra, Chakib Arsalane Street, Kénitra (Morocco); Jorio, Anouar; Zorkani, Izeddine [LPS, Faculty of sciences, Dhar EL Mehrez, B.P 1796 Atlas Fez (Morocco)
2013-07-15
Within the framework of the effective mass scheme, the ground-state binding energy of hydrogenic shallow-donor impurity in wurtzite (WZ) (In,Ga)N/GaN parabolic transversal-section quantum-well wire (PQWW) subjected to magnetic field is investigated. The finite-difference method within the quasi-one-dimensional effective potential model is used. A cylindrical QWW effective radius is introduced to describe the lateral confinement strength. The results show that: (i) the binding energy is the largest for the impurity located at a point corresponding to the largest electron probability density and (ii) it increases with increasing external magnetic field.
Dirac Fermions in an Antiferromagnetic Semimetal
Tang, Peizhe; Zhou, Quan; Xu, Gang; Zhang, Shou-Cheng; Shou-Cheng Zhang's Group Team, Prof.
Analogues of the elementary particles have been extensively searched for in condensed matter systems for both scientific interest and technological applications. Recently, massless Dirac fermions were found to emerge as low energy excitations in materials now known as Dirac semimetals. All the currently known Dirac semimetals are nonmagnetic with both time-reversal symmetry and inversion symmetry "". Here we show that Dirac fermions can exist in one type of antiferromagnetic systems, where both and "" are broken but their combination "" is respected. We propose orthorhombic antiferromagnet CuMnAs as a candidate, analyze the robustness of the Dirac points under symmetry protections, and demonstrate its distinctive bulk dispersions as well as the corresponding surface states by ab initio calculations. Our results provide a possible platform to study the interplay of Dirac fermion physics and magnetism. We acknowledge the DOE, Office of Basic Energy Sciences, Division of Materials Sciences and Engineering, under contract DE-AC02-76SF00515, NSF under Grant No.DMR-1305677 and FAME, one of six centers of STARnet.
Magnetic properties of TMCuC : Mn, a quantum chain with classical impurities
International Nuclear Information System (INIS)
Dupas, C.; Renard, J.P.; Seiden, J.; Cheikh-Rouhou, A.
1981-01-01
The magnetic susceptibility of the mixed quasi one-dimensional system (CH 3 ) 4 NMnsub(x)Cusub(1-x) has been measured down to 0.32 K for x ranging between 0 an 1. At 4.2 K, the susceptibility starts to increase with x up to x = 0.1 and then decreases rapidly. The Neel temperature decreases from 1.24 K for x = 0 to 0.35 K for x = 0.22. The experimental data at small values of x are well explained by a theoretical model of S = 1/2 quantum chain with classical impurities. (orig.)
Single-site approximation for the s-f model of antiferromagnetic semiconductors
International Nuclear Information System (INIS)
Takahashi, Masao; Nolting, Wolfgang
2001-01-01
For the s-f model of an antiferromagnetic semiconductor, the effect of the antiferromagnetic ordering of the localized spins on the conduction-electron state is investigated over a wide range of exchange strengths by combining the effective-medium approach with the Green's function in the 2x2 sublattice Bloch function representation. The band splitting due to the reduced magnetic Brillouin zone occurs below the Neel temperature. There is a marked effect of the thermal fluctuation of the antiferromagnetically ordered localized spins on the conduction electron at the energies near the top (bottom) of the lower- (higher-) energy subband
Quasi One-Dimensional Model of Natural Draft Wet-Cooling Tower Flow, Heat and Mass Transfer
Directory of Open Access Journals (Sweden)
Hyhlík Tomáš
2015-01-01
Full Text Available The article deals with the development of CFD (Computational Fluid Dynamics model of natural draft wet-cooling tower flow, heat and mass transfer. The moist air flow is described by the system of conservation laws along with additional equations. Moist air is assumed to be homogeneous mixture of dry air and water vapour. Liquid phase in the fill zone is described by the system of ordinary differential equations. Boundary value problem for the system of conservation laws is discretized in space using Kurganov-Tadmor central scheme and in time using strong stability preserving Runge-Kutta scheme. Initial value problems in the fill zone is solved by using standard fourth order Runge-Kutta scheme. The interaction between liquid water and moist air is done by source terms in governing equations.
International Nuclear Information System (INIS)
Mugge, J.W.
1979-10-01
The collisional plasma transport problem is formulated as an initial boundary value problem for general characteristic boundary conditions. Starting from the full set of hydrodynamic and electrodynamic equations an expansion in the electron-ion mass ratio together with a multiple timescale method yields simplified equations on each timescale. On timescales where many collisions have taken place for the simplified equations the initial boundary value problem is formulated. Through the introduction of potentials a two-dimensional scalar formulation in terms of quasi-linear integro-differential equations of second order for a domain consisting of plasma and vacuum sub-domains is obtained. (Auth.)
Dessup, Tommy; Coste, Christophe; Saint Jean, Michel
2017-01-01
We study the path toward equilibrium of pairs of solitary wave envelopes (bubbles) that modulate a regular zigzag pattern in an annular channel. We evidence that bubble pairs are metastable states, which spontaneously evolve toward a stable single bubble. We exhibit the concept of topological frustration of a bubble pair. A configuration is frustrated when the particles between the two bubbles are not organized in a modulated staggered row. For a nonfrustrated (NF) bubble pair configuration, the bubbles interaction is attractive, whereas it is repulsive for a frustrated (F) configuration. We describe a model of interacting solitary wave that provides all qualitative characteristics of the interaction force: It is attractive for NF systems and repulsive for F systems and decreases exponentially with the bubbles distance. Moreover, for NF systems, the bubbles come closer and eventually merge as a single bubble, in a coalescence process. We also evidence a collapse process, in which one bubble shrinks in favor of the other one, overcoming an energetic barrier in phase space. This process is relevant for both NF systems and F systems. In NF systems, the coalescence prevails at low temperature, whereas thermally activated jumps make the collapse prevail at high temperature. In F systems, the path toward equilibrium involves a collapse process regardless of the temperature.
Czech Academy of Sciences Publication Activity Database
Yulin, A.V.; Bludov, Yu.V.; Konotop, V. V.; Kuzmiak, Vladimír; Salerno, M.
2013-01-01
Roč. 87, č. 3 (2013) ISSN 1050-2947 R&D Projects: GA MŠk LH12009 Institutional support: RVO:67985882 Keywords : Superfluidity * Bose-Einstein condensates * Matter Waves Subject RIV: JA - Electronics ; Optoelectronics, Electrical Engineering Impact factor: 2.991, year: 2013
Exchange bias in diluted-antiferromagnet/antiferromagnet bilayers
International Nuclear Information System (INIS)
Mao, Zhongquan; Zhan, Xiaozhi; Chen, Xi
2015-01-01
The hysteresis-loop properties of a diluted-antiferromagnetic (DAF) layer exchange coupling to an antiferromagnetic (AF) layer are investigated by means of numerical simulations. Remarkable loop shift and coercivity enhancement are observed in such DAF/AF bilayers, while they are absent in the uncoupled DAF single layer. The influences of pinned domains, dilution, cooling field and DAF layer thickness on the loop shift are investigated systematically. The result unambiguously confirms an exchange bias (EB) effect in the DAF/AF bilayers. It also reveals that the EB effect originates from the pinned AF domains within the DAF layer. In contrast to conventional EB systems, frozen uncompensated spins are not found at the interface of the AF pinning layer. (paper)
Competing interactions in ferromagnetic/antiferromagnetic perovskite superlattices
Energy Technology Data Exchange (ETDEWEB)
Takamura, Y.; Biegalski, M.B.; Christen, H.M.
2009-10-22
Soft x-ray magnetic dichroism, magnetization, and magnetotransport measurements demonstrate that the competition between different magnetic interactions (exchange coupling, electronic reconstruction, and long-range interactions) in La{sub 0.7}Sr{sub 0.3}FeO{sub 3}(LSFO)/La{sub 0.7}Sr{sub 0.3}MnO{sub 3}(LSMO) perovskite oxide superlattices leads to unexpected functional properties. The antiferromagnetic order parameter in LSFO and ferromagnetic order parameter in LSMO show a dissimilar dependence on sublayer thickness and temperature, illustrating the high degree of tunability in these artificially layered materials.
Collective impurity effects in the Heisenberg triangular antiferromagnet
International Nuclear Information System (INIS)
Maryasin, V S; Zhitomirsky, M E
2015-01-01
We theoretically investigate the Heisenberg antiferromagnet on a triangular lattice doped with nonmagnetic impurities. Two nontrivial effects resulting from collective impurity behavior are predicted. The first one is related to presence of uncompensated magnetic moments localized near vacancies as revealed by the low-temperature Curie tail in the magnetic susceptibility. These moments exhibit an anomalous growth with the impurity concentration, which we attribute to the clustering mechanism. In an external magnetic field, impurities lead to an even more peculiar phenomenon lifting the classical ground-state degeneracy in favor of the conical state. We analytically demonstrate that vacancies spontaneously generate a positive biquadratic exchange, which is responsible for the above degeneracy lifting
Antiferromagnetic exchange coupling measurements on single Co clusters
Wernsdorfer, W.; Leroy, D.; Portemont, C.; Brenac, A.; Morel, R.; Notin, L.; Mailly, D.
2009-03-01
We report on single-cluster measurements of the angular dependence of the low-temperature ferromagnetic core magnetization switching field in exchange-coupled Co/CoO core-shell clusters (4 nm) using a micro-bridge DC superconducting quantum interference device (μ-SQUID). It is observed that the coupling with the antiferromagnetic shell induces modification in the switching field for clusters with intrinsic uniaxial anisotropy depending on the direction of the magnetic field applied during the cooling. Using a modified Stoner-Wohlfarth model, it is shown that the core interacts with two weakly coupled and asymmetrical antiferromagnetic sublattices. Ref.: C. Portemont, R. Morel, W. Wernsdorfer, D. Mailly, A. Brenac, and L. Notin, Phys. Rev. B 78, 144415 (2008)
Energy Technology Data Exchange (ETDEWEB)
Ikeda, H; Suzuki, M [Ochanomizu Univ., Tokyo (Japan). Dept. of Physics; Hutchings, M T [UKAEA Atomic Energy Research Establishment, Harwell. Materials Physics Div.
1979-01-01
The spin correlation between two-dimensionally (2D) ordered antiferromagnetic layers in the random antiferromagnets Rb/sub 2/Cosub(c)Mgsub(1-c)F/sub 4/ depends strongly on the rate at which the sample is cooled through the Neel point Tsub(N) and decreases markedly with decreasing Co/sup 2 +/ ion concentration c. Preliminary data are presented which indicate that the order below sub(N) is metastable and relaxes to a fully correlated 3D ordered state on a finite, measurable, time-scale.
Antiferromagnetic ordering of Er2NiSi3 compound
International Nuclear Information System (INIS)
Pakhira, Santanu; Mazumdar, Chandan; Ranganathan, R.
2014-01-01
Ternary intermetallics of the stoichiometric composition R 2 TX 3 , where, R = rare earth element, T = d-electron transition metal and X= p-electron element, crystallizes in hexagonal A1B 2 type crystal structure with space group P6/mmm. We report here the synthesis and basic magnetic properties of the compound Er 2 NiSi 3 . Paramagnetic to antiferromagnetic phase change occurs below 5.4 K for this compound. (author)
Spintronic materials and devices based on antiferromagnetic metals
Wang, Y.Y.; Song, C.; Zhang, J.Y.; Pan, F.
2017-01-01
In this paper, we review our recent experimental developments on antiferromagnet (AFM) spintronics mainly comprising Mn-based noncollinear AFM metals. IrMn-based tunnel junctions and Hall devices have been investigated to explore the manipulation of AFM moments by magnetic fields, ferromagnetic materials and electric fields. Room-temperature tunneling anisotropic magnetoresistance based on IrMn as well as FeMn has been successfully achieved, and electrical control of the AFM exchange spring i...
Isothermal anisotropic magnetoresistance in antiferromagnetic metallic IrMn
Czech Academy of Sciences Publication Activity Database
Galceran, R.; Fina, I.; Cisneros-Fernandez, J.; Bozzo, B.; Frontera, C.; Lopez-Mir, L.; Deniz, H.; Park, K.W.; Park, B.G.; Balcells, J.; Martí, Xavier; Jungwirth, Tomáš; Martínez, B.
2016-01-01
Roč. 6, Oct (2016), 1-6, č. článku 35471. ISSN 2045-2322 R&D Projects: GA MŠk LM2015087; GA ČR GB14-37427G EU Projects: European Commission(XE) 268066 - 0MSPIN Institutional support: RVO:68378271 Keywords : antiferromagnets * spintronics * magnetoresistance Subject RIV: BM - Solid Matter Physics ; Magnetism Impact factor: 4.259, year: 2016
Analogies between antiferromagnets and antiferroelectrics
International Nuclear Information System (INIS)
Enz, C.P.; Matthias, B.T.
1980-01-01
Ferro- and antiferromagnetism in the Laves phase TiBesub(2-x) Cusub(x) occurs for 0.1 4 H 2 PO 4 and its solid solutions with TlH 2 PO 4 and with the ferroelectric KH 2 PO 4 are discussed as function of deuteration and of pressure. Another analogy as function of pressure is established with the antiferroelectric perovskite PbZrO 3 . (author)
Weyl magnons in noncoplanar stacked kagome antiferromagnets
Owerre, S. A.
2018-03-01
Weyl nodes have been experimentally realized in photonic, electronic, and phononic crystals. However, magnonic Weyl nodes are yet to be seen experimentally. In this paper, we propose Weyl magnon nodes in noncoplanar stacked frustrated kagome antiferromagnets, naturally available in various real materials. Most crucially, the Weyl nodes in the current system occur at the lowest excitation and possess a topological thermal Hall effect, therefore they are experimentally accessible at low temperatures due to the population effect of bosonic quasiparticles. In stark contrast to other magnetic systems, the current Weyl nodes do not rely on time-reversal symmetry breaking by the magnetic order. Rather, they result from explicit macroscopically broken time reversal symmetry by the scalar spin chirality of noncoplanar spin textures and can be generalized to chiral spin liquid states. Moreover, the scalar spin chirality gives a real space Berry curvature which is not available in previously studied magnetic Weyl systems. We show the existence of magnon arc surface states connecting projected Weyl magnon nodes on the surface Brillouin zone. We also uncover the first realization of triply-degenerate nodal magnon point in the noncollinear regime with zero scalar spin chirality.
Spin diffusion and torques in disordered antiferromagnets
Manchon, Aurelien
2017-02-01
We have developed a drift-diffusion equation of spin transport in collinear bipartite metallic antiferromagnets. Starting from a model tight-binding Hamiltonian, we obtain the quantum kinetic equation within Keldysh formalism and expand it to the lowest order in spatial gradient using Wigner expansion method. In the diffusive limit, these equations track the spatio-temporal evolution of the spin accumulations and spin currents on each sublattice of the antiferromagnet. We use these equations to address the nature of the spin transfer torque in (i) a spin-valve composed of a ferromagnet and an antiferromagnet, (ii) a metallic bilayer consisting of an antiferromagnet adjacent to a heavy metal possessing spin Hall effect, and in (iii) a single antiferromagnet possessing spin Hall effect. We show that the latter can experience a self-torque thanks to the non-vanishing spin Hall effect in the antiferromagnet.
Spin diffusion and torques in disordered antiferromagnets
Manchon, Aurelien
2017-01-01
We have developed a drift-diffusion equation of spin transport in collinear bipartite metallic antiferromagnets. Starting from a model tight-binding Hamiltonian, we obtain the quantum kinetic equation within Keldysh formalism and expand it to the lowest order in spatial gradient using Wigner expansion method. In the diffusive limit, these equations track the spatio-temporal evolution of the spin accumulations and spin currents on each sublattice of the antiferromagnet. We use these equations to address the nature of the spin transfer torque in (i) a spin-valve composed of a ferromagnet and an antiferromagnet, (ii) a metallic bilayer consisting of an antiferromagnet adjacent to a heavy metal possessing spin Hall effect, and in (iii) a single antiferromagnet possessing spin Hall effect. We show that the latter can experience a self-torque thanks to the non-vanishing spin Hall effect in the antiferromagnet.
Spin Wave Theory in Two-Dimensional Coupled Antiferromagnets
Shimahara, Hiroshi
2018-04-01
We apply spin wave theory to two-dimensional coupled antiferromagnets. In particular, we primarily examine a system that consists of small spins coupled by a strong exchange interaction J1, large spins coupled by a weak exchange interaction J2, and an anisotropic exchange interaction J12 between the small and large spins. This system is an effective model of the organic antiferromagnet λ-(BETS)2FeCl4 in its insulating phase, in which intriguing magnetic phenomena have been observed, where the small and large spins correspond to π electrons and 3d spins, respectively. BETS stands for bis(ethylenedithio)tetraselenafulvalene. We obtain the antiferromagnetic transition temperature TN and the sublattice magnetizations m(T) and M(T) of the small and large spins, respectively, as functions of the temperature T. When T increases, m(T) is constant with a slight decrease below TN, even where M(T) decreases significantly. When J1 ≫ J12 and J2 = 0, an analytical expression for TN is derived. The estimated value of TN and the behaviors of m(T) and M(T) agree with the observations of λ-(BETS)2FeCl4.
Microscopic theory of coexistence of superconductivity and antiferromagnetism
International Nuclear Information System (INIS)
Ashkenazi, J.; Kuper, C.G.; Ron, A.
1983-01-01
A theory of the coexistence of superconductivity and antiferromagnetism is presented. We study the role of the ''diagonal'' exchange coupling between magnetic ions and conduction electrons, using Eliashberg's formalism. This coupling generates a spatial displacement of the Cooper-paired states, and thus reduces the pairing strength. The reduction is linear in the exchange integral and the staggered magnetization. The theory agrees well with experiment for Dy/sub 1.2/Mo 6 S 8 and Tb/sub 1.2/Mo 6 S 8
Crystal structure and magnetic properties of the solid-solution phase Ca3Co2-v Sc v O6
International Nuclear Information System (INIS)
Hervoches, Charles H.; Fredenborg, Vivian Miksch; Kjekshus, Arne; Fjellvag, Helmer; Hauback, Bjorn C.
2007-01-01
The two crystallographically non-equivalent Co atoms of the quasi-one-dimensional crystal structure of Ca 3 Co 2 O 6 form chains with alternating, face-sharing polyhedra of Co2O 6 trigonal prisms and Co1O 6 octahedra. This compound forms a substitutional solid-solution phase with Sc, in which the Sc atoms enter the Co2 sublattice exclusively. The homogeneity range of Ca 3 Co 2- v Sc v O 6 (more specifically Ca 3 Co1Co2 1- v Sc v O 6 ) extends up to v∼0.55. The crystal structure belongs to space group R3-barc with lattice parameters (in hexagonal setting): 9.0846(3)≤a≤9.1300(2) A and 10.3885(4)≤c≤10.4677(4) A. The magnetic moment decreases rapidly with increasing amount of the non-magnetic Sc solute in the lattice. - Graphical abstract: The quasi-one-dimensional Ca 3 Co 2 O 6 phase forms a substitutional solid-solution system with Sc, in which the Sc atoms enter the Co2 sublattice exclusively. The homogeneity range of Ca 3 Co 2- v Sc v O 6 extends up to v∼0.55. The magnetic moment decreases rapidly with increasing amount of the non-magnetic Sc solute in the lattice
Energy Technology Data Exchange (ETDEWEB)
Qiu, Rong-ke, E-mail: rkqiu@163.com; Cai, Wei
2017-08-15
Highlights: • A quantum approach is developed to study the SWR of a bicomponent multi-layer films. • The comparison of the SWR in films with FM and AFM interfacial coupling has been made. • The present results show the method to enhance and adjust the SWR frequency of films. - Abstract: We investigate the spin-wave resonance (SWR) frequency in a bicomponent bilayer and triple-layer films with antiferromagnetic or ferromagnetic interfacial couplings, as function of interfacial coupling, surface anisotropy, interface anisotropy, thickness and external magnetic field, using the linear spin-wave approximation and Green’s function technique. The microwave properties for multi-layer magnetic film with antiferromagnetic interfacial coupling is different from those for multi-layer magnetic film with ferromagnetic interfacial coupling. For the bilayer film with antiferromagnetic interfacial couplings, as the lower (upper) surface anisotropy increases, only the SWR frequencies of the odd (even) number modes increase. The lower (upper) surface anisotropy does not affect the SWR frequencies of the even (odd) number modes{sub .} For the multi-layer film with antiferromagnetic interfacial coupling, the SWR frequency of modes m = 1, 3 and 4 decreases while that of mode m = 2 increases with increasing thickness of the film within a proper parameter region. The present results could be useful in enhancing our fundamental understanding and show the method to enhance and adjust the SWR frequency of bicomponent multi-layer magnetic films with antiferromagnetic or ferromagnetic interfacial coupling.
Soft modes in the easy plane pyrochlore antiferromagnet
International Nuclear Information System (INIS)
Champion, J D M; Holdsworth, P C W
2004-01-01
Thermal fluctuations lift the high ground state degeneracy of the classical nearest neighbour pyrochlore antiferromagnet, with easy plane anisotropy, giving a first-order phase transition to a long range ordered state. We show, from spin wave analysis and numerical simulation, that even below this transition a continuous manifold of states, of dimension N 2/3 , exist (N is the number of degrees of freedom). As the temperature goes to zero a further 'order by disorder' selection is made from this manifold. The pyrochlore antiferromagnet Er 2 Ti 2 O 7 is believed to have an easy plane anisotropy and is reported to have the same magnetic structure. This is perhaps surprising, given that the dipole interaction lifts the degeneracy of the classical model in favour of a different structure. We interpret our results in the light of these facts
Spiral phases of doped antiferromagnets
International Nuclear Information System (INIS)
Shraiman, B.I.; Siggia, E.D.
1990-01-01
The dipole density field describing the holls in a doped antiferromagnet is considered for law hole density in the semiclassical limit. This yields a phase in which the order parameter is planar and spirals round a fixed direction. The single spiral state breaks the continuous spin rotational symmetry and exhibits long-range order at zero temperature. In it there is a global spin direction as rotation axis. The double spiral state, in which there are two perpendicular directions, is isotropic in both spin and real space. Several results of microscopic calculations, carried out to understand the electronic states, quantum fluctuations, lattice effects and normal mode dynamics, are recapitulated. 8 refs
Antiferromagnetism and magnetoleasticity of UNiAl
International Nuclear Information System (INIS)
Sechovsky, V.; Honda, F.; Svoboda, P.; Prokes, K.; Chernyavsky, O.; Doerr, M.; Rotter, M.; Loewenhaupt, M.
2003-01-01
We report on a thermal-expansion (TE) and magnetostriction (MS) study of the antiferromagnet UNiAl at temperatures 2-90 K and in magnetic fields up to 16.5 T applied along the c-axis. The TE along the c-axis (in 0 T) exhibits a broad valley centered around 35 K. This anomaly is nearly removed in 16.5 T. For T≤7 K a sharp metamagnetic transition (MT) observed in UNiAl at 11.4 T and it is accompanied by abrupt MS effects of +1.3x10 -4 and -1.8x10 -4 along the a- and c-axis, respectively. In fields above the MT a negligible additional negative MS is induced along c-axis whereas the a-axis and consequently the volume expand considerably, which indicates a field-induced enhancement of the U magnetic moment. T>7 K, the MT becomes gradually smeared out but a non-negligible MS is observed even for T>T N . In the light of these results the TE anomaly measured in zero field may be attributed to AF that survives at temperatures far above T N
Antiferromagnetic Skyrmion: Stability, Creation and Manipulation
Zhang, Xichao; Zhou, Yan; Ezawa, Motohiko
2016-04-01
Magnetic skyrmions are particle-like topological excitations in ferromagnets, which have the topo-logical number Q = ± 1, and hence show the skyrmion Hall effect (SkHE) due to the Magnus force effect originating from the topology. Here, we propose the counterpart of the magnetic skyrmion in the antiferromagnetic (AFM) system, that is, the AFM skyrmion, which is topologically protected but without showing the SkHE. Two approaches for creating the AFM skyrmion have been described based on micromagnetic lattice simulations: (i) by injecting a vertical spin-polarized current to a nanodisk with the AFM ground state; (ii) by converting an AFM domain-wall pair in a nanowire junction. It is demonstrated that the AFM skyrmion, driven by the spin-polarized current, can move straightly over long distance, benefiting from the absence of the SkHE. Our results will open a new strategy on designing the novel spintronic devices based on AFM materials.
International Nuclear Information System (INIS)
Fernández-Pacheco, A.; Mansell, R.; Petit, D.; Lee, J. H.; Cowburn, R. P.; Ummelen, F. C.; Swagten, H. J. M.
2014-01-01
We have designed a bilayer synthetic antiferromagnet where the order of layer reversal can be selected by varying the sweep rate of the applied magnetic field. The system is formed by two ultra-thin ferromagnetic layers with different proximities to the spin reorientation transition, coupled antiferromagnetically using Ruderman-Kittel-Kasuya-Yosida interactions. The different dynamic magnetic reversal behavior of both layers produces a crossover in their switching fields for field rates in the kOe/s range. This effect is due to the different effective anisotropy of both layers, added to an appropriate asymmetric antiferromagnetic coupling between them. Field-rate controlled selective switching of perpendicular magnetic anisotropy layers as shown here can be exploited in sensing and memory applications.
Energy Technology Data Exchange (ETDEWEB)
Cinti, F. [INFM and Department of Physics, University of Florence, 50019 Sesto Fiorentino (Italy)]. E-mail: fabio.cinti@fi.infn.it; Rettori, A. [INFM and Department of Physics, University of Florence, 50019 Sesto Fiorentino (Italy); Barucci, M. [INFM and Department of Physics, University of Florence, 50019 Sesto Fiorentino (Italy); Olivieri, E. [INFM and Department of Physics, University of Florence, 50019 Sesto Fiorentino (Italy); Risegari, L. [INFM and Department of Physics, University of Florence, 50019 Sesto Fiorentino (Italy); Ventura, G. [INFM and Department of Physics, University of Florence, 50019 Sesto Fiorentino (Italy); Caneschi, A. [Department of Inorganic Chemistry, University of Florence, 50019 Sesto Fiorentino (Italy); Gatteschi, D. [Department of Inorganic Chemistry, University of Florence, 50019 Sesto Fiorentino (Italy); Rovai, D. [Department of Inorganic Chemistry, University of Florence, 50019 Sesto Fiorentino (Italy); Pini, M.G. [ISC-CNR, 50019 Sesto Fiorentino (Italy); Affronte, M. [INFM-S3 and Department of Physics, University of Modena, 41100 Modena (Italy); Mariani, M. [INFM and Department of Physics, University of Pavia, 27100 Pavia (Italy); Lascialfari, A. [Istituto di Fisiologia e Chimica Biologica, University of Milano, Milano (Italy); INFM and Department of Physics, University of Pavia, 27100 Pavia (Italy)
2007-03-15
New specific heat data taken at very low temperatures (0.03
Precessional switching of antiferromagnets by electric field induced Dzyaloshinskii-Moriya torque
Kim, T. H.; Grünberg, P.; Han, S. H.; Cho, B. K.
2018-05-01
Antiferromagnetic insulators (AFIs) have attracted much interest from many researchers as promising candidates for use in ultrafast, ultralow-dissipation spintronic devices. As a fast method of reversing magnetization, precessional switching is realized when antiferromagnetic Néel orders l =(s1+s2 )/2 surmount the magnetic anisotropy or potential barrier in a given magnetic system, which is described well by the antiferromagnetic plane pendulum (APP) model. Here, we report that, as an alternative switching scenario, the direct coupling of an electric field with Dzyaloshinskii-Moriya (DM) interaction, which stems from spin-orbit coupling, is exploited for optimal switching. We derive the pendulum equation of motion of antiferromagnets, where DM torque is induced by a pulsed electric field. The temporal DM interaction is found to not only be in the form of magnetic torques (e.g., spin-orbit torque or magnetic field) but also modifies the magnetic potential that limits l 's activity; as a result, appropriate controls (e.g., direction, magnitude, and pulse shape) of the induced DM vector realize deterministic reversal in APP. The results present an approach for the control of a magnetic storage device by means of an electric field.
The Heisenberg antiferromagnet on the square-kagomé lattice
Directory of Open Access Journals (Sweden)
J. Richter
2009-01-01
Full Text Available We discuss the ground state, the low-lying excitations as well as high-field thermodynamics of the Heisenberg antiferromagnet on the two-dimensional square-kagomé lattice. This magnetic system belongs to the class of highly frustrated spin systems with an infinite non-trivial degeneracy of the classical ground state as it is also known for the Heisenberg antiferromagnet on the kagomé and on the star lattice. The quantum ground state of the spin-half system is a quantum paramagnet with a finite spin gap and with a large number of non-magnetic excitations within this gap. We also discuss the magnetization versus field curve that shows a plateaux as well as a macroscopic magnetization jump to saturation due to independent localized magnon states. These localized states are highly degenerate and lead to interesting features in the low-temperature thermodynamics at high magnetic fields such as an additional low-temperature peak in the specific heat and an enhanced magnetocaloric effect.
Spin-orbit torque in two-dimensional antiferromagnetic topological insulators
Ghosh, Sumit; Manchon, Aurelien
2017-01-01
We investigate spin transport in two-dimensional ferromagnetic (FTI) and antiferromagnetic (AFTI) topological insulators. In the presence of an in-plane magnetization AFTI supports zero energy modes, which enables topologically protected edge conduction at low energy. We address the nature of current-driven spin torque in these structures and study the impact of spin-independent disorder. Interestingly, upon strong disorder the spin torque develops an antidamping component (i.e., even upon magnetization reversal) along the edges, which could enable current-driven manipulation of the antiferromagnetic order parameter. This antidamping torque decreases when increasing the system size and when the system enters the trivial insulator regime.
Controlling the switching field in nanomagnets by means of domain-engineered antiferromagnets
Folven, E.; Linder, J.; Gomonay, O. V.; Scholl, A.; Doran, A.; Young, A. T.; Retterer, S. T.; Malik, V. K.; Tybell, T.; Takamura, Y.; Grepstad, J. K.
2015-09-01
Using soft x-ray spectromicroscopy, we investigate the magnetic domain structure in embedded nanomagnets defined in L a0.7S r0.3Mn O3 thin films and LaFe O3/L a0.7S r0.3Mn O3 bilayers. We find that shape-controlled antiferromagnetic domain states give rise to a significant reduction of the switching field of the rectangular nanomagnets. This is discussed within the framework of competition between an intrinsic spin-flop coupling and shape anisotropy. The data demonstrates that shape effects in antiferromagnets may be used to control the magnetic properties in nanomagnets.
Antiferromagnetism and its relation to the superconducting phases of UPt3
DEFF Research Database (Denmark)
Isaacs, E.D.; Zschack, P.; Broholm, C.L.
1995-01-01
Using magnetic x-ray and neutron diffraction in UPt3, we find that a suppression of the antiferromagnetic scattering intensity in the superconducting phase is due to a reduction in the magnitude of the staggered moment with no change in symmetry. The existence of the suppression as well...... as the magnetic correlation lengths are not affected by the presence or absence of a visible splitting in the superconducting transition. The simplest models wherein antiferromagnetic order provides the symmetry-breaking field for the splitting do not provide a compete explanation of our results....
Spin-orbit torque in two-dimensional antiferromagnetic topological insulators
Ghosh, Sumit
2017-01-24
We investigate spin transport in two-dimensional ferromagnetic (FTI) and antiferromagnetic (AFTI) topological insulators. In the presence of an in-plane magnetization AFTI supports zero energy modes, which enables topologically protected edge conduction at low energy. We address the nature of current-driven spin torque in these structures and study the impact of spin-independent disorder. Interestingly, upon strong disorder the spin torque develops an antidamping component (i.e., even upon magnetization reversal) along the edges, which could enable current-driven manipulation of the antiferromagnetic order parameter. This antidamping torque decreases when increasing the system size and when the system enters the trivial insulator regime.
Antiferromagnetism in EuPdGe{sub 3}
Energy Technology Data Exchange (ETDEWEB)
Albedah, Mohammed A. [Department of Physics, University of Ottawa, Ottawa, Ontario K1N 6N5 (Canada); Al-Qadi, Khalid [Department of Physics, University of Ottawa, Ottawa, Ontario K1N 6N5 (Canada); Department of Mathematics, Statistics and Physics, Qatar University, P.O. Box 2713, Doha (Qatar); Stadnik, Zbigniew M., E-mail: stadnik@uottawa.ca [Department of Physics, University of Ottawa, Ottawa, Ontario K1N 6N5 (Canada); Przewoźnik, Janusz [Solid State Physics Department, Faculty of Physics and Applied Computer Science, AGH University of Science and Technology, 30-059 Kraków (Poland)
2014-11-15
Highlights: • We show that EuPdGe{sub 3} crystallizes in the BaNiSn{sub 3}-type structure with the lattice constants a = 4.4457(1) Å and c = 10.1703(2). • We demonstrate that EuPdGe{sub 3} is an antiferromagnet with the Néel temperature T{sub N} = 12.16(1) K. • The temperature dependence of the hyperfine magnetic field follows a S = 7/2 Brillouin function. • We find that the Debye temperature of the studied compound is 199(2) K. - Abstract: The results of X-ray diffraction, magnetic susceptibility and magnetization, and {sup 151}Eu Mössbauer spectroscopy measurements of polycrystalline EuPdGe{sub 3} are reported. EuPdGe{sub 3} crystallizes in the BaNiSn{sub 3}-type tetragonal structure (space group I4mm) with the lattice constants a=4.4457(1)Å and c=10.1703(2)Å. The results are consistent with EuPdGe{sub 3} being an antiferromagnet with the Néel temperature T{sub N}=12.16(1)K and with the Eu spins S=7/2 in the ab plane. The temperature dependence of the magnetic susceptibility above T{sub N} follows the modified Curie-Weiss law with the effective magnetic moment of 7.82(1) μ{sub B} per Eu atom and the paramagnetic Curie temperature of -5.3(1)K indicative of dominant antiferromagnetic interactions. The M(H) isotherms for temperatures approaching T{sub N} from above are indicative of dynamical short-range antiferromagnetic ordering in the sample. The temperature dependence of the hyperfine magnetic field follows a S=7/2 Brillouin function. The principal component of the electric field gradient tensor is shown to increase with decreasing temperature and is well described by a T{sup 3/2} power-law relation. The Debye temperature of EuPdGe{sub 3} determined from the Mössbauer data is 199(2) K.
Orbital and magnetic structure of quasi-1D cobaltites: Ab initio calculations and experiment
International Nuclear Information System (INIS)
Pardo, V.; Baldomir, D.; Rivas, J.; Castro, J.; Arias, J.E.
2006-01-01
The magnetic properties of the orbitally degenerate quasi-one-dimensional cobaltites Sr x Ba 1-x CoO 3 are explained on the basis of a phase separation phenomenon. Noninteracting magnetic particles embedded in a nonferromagnetic matrix develop in the system. Details are given about the electronic and magnetic structure for x=0,0.2 and 0.5. At x=0.5, the geometry of the CoO 6 trigonally distorted octahedra changes by about 1-2%, but magnetic particles get 3 times bigger, compared to the parent compound, with the corresponding changes in the magnetic properties. The electronic structure of the Co 4+ ion, however, stays roughly unchanged
Low-frequency response in antiferromagnetically coupled Fe/Cr multilayers
International Nuclear Information System (INIS)
Aliev, F.G.; Guerrero, R.; Martinez, J.L.; Moshchalkov, V.V.; Bruynseraede, Y.; Villar, R.
2001-01-01
We have studied the magnetic field dependences of the real (χ) and imaginary (χ') contributions to the low-frequency magnetic susceptibility in epitaxial antiferromagnetically coupled [Fe(Cr(1 0 0)] n (n=10-50) multilayers. For the magnetic field directed along (1 1 0), the magnetic susceptibility shows on orientation phase transition. For the magnetic field either along the easy or the hard axes we observe a strong enhancement of the χ'(H) (i.e. magnetic losses) at low magnetic fields (H<50 Oe), which we relate to AC field-induced domain wall movement. This response is strongly dependent on frequency and temperature
Antiferromagnetic order in the Hubbard model on the Penrose lattice
Koga, Akihisa; Tsunetsugu, Hirokazu
2017-12-01
We study an antiferromagnetic order in the ground state of the half-filled Hubbard model on the Penrose lattice and investigate the effects of quasiperiodic lattice structure. In the limit of infinitesimal Coulomb repulsion U →+0 , the staggered magnetizations persist to be finite, and their values are determined by confined states, which are strictly localized with thermodynamics degeneracy. The magnetizations exhibit an exotic spatial pattern, and have the same sign in each of cluster regions, the size of which ranges from 31 sites to infinity. With increasing U , they continuously evolve to those of the corresponding spin model in the U =∞ limit. In both limits of U , local magnetizations exhibit a fairly intricate spatial pattern that reflects the quasiperiodic structure, but the pattern differs between the two limits. We have analyzed this pattern change by a mode analysis by the singular value decomposition method for the fractal-like magnetization pattern projected into the perpendicular space.
Helical waves in easy-plane antiferromagnets
Semenov, Yuriy G.; Li, Xi-Lai; Xu, Xinyi; Kim, Ki Wook
2017-12-01
Effective spin torques can generate the Néel vector oscillations in antiferromagnets (AFMs). Here, it is theoretically shown that these torques applied at one end of a normal AFM strip can excite a helical type of spin wave in the strip whose properties are drastically different from characteristic spin waves. An analysis based on both a Néel vector dynamical equation and the micromagnetic simulation identifies the direction of magnetic anisotropy and the damping factor as the two key parameters determining the dynamics. Helical wave propagation requires the hard axis of the easy-plane AFM to be aligned with the traveling direction, while the damping limits its spatial extent. If the damping is neglected, the calculation leads to a uniform periodic domain wall structure. On the other hand, finite damping decelerates the helical wave rotation around the hard axis, ultimately causing stoppage of its propagation along the strip. With the group velocity staying close to spin-wave velocity at the wave front, the wavelength becomes correspondingly longer away from the excitation point. In a sufficiently short strip, a steady-state oscillation can be established whose frequency is controlled by the waveguide length as well as the excitation energy or torque.
Quantum disordered phase in a doped antiferromagnet
International Nuclear Information System (INIS)
Kuebert, C.; Muramatsu, A.
1995-01-01
A quantitative description of the transition to a quantum disordered phase in a doped antiferromagnet is obtained for the long-wavelength limit of the spin-fermion model, which is given by the O(3) non-linear σ model, a free fermionic part and current-current interactions. By choosing local spin quantization axes for the fermionic spinor we show that the low-energy limit of the model is equivalent to a U(1) gauge theory, where both the bosonic and fermionic degrees of freedom are minimally coupled to a vector gauge field. Within a large-N expansion, the strength of the gauge fields is found to be determined by the gap in the spin-wave spectrum, which is dynamically generated. The explicit doping dependence of the spin-gap is determined as a function of the parameters of the original model. As a consequence of the above, the gauge-fields mediate a long-range interaction among dopant holes and S-1/2 magnetic excitations only in the quantum disordered phase. The possible bound-states in this regime correspond to charge-spin separation and pairing
Lebyodkin, M. A.; Lebedkina, T. A.; Shashkov, I. V.; Gornakov, V. S.
2017-07-01
Magnetization reversal of polycrystalline NiFe/NiO bilayers was investigated using magneto-optical indicator film imaging and acoustic emission techniques. Sporadic acoustic signals were detected in a constant magnetic field after the magnetization reversal. It is suggested that they are related to elastic waves excited by sharp shocks in the NiO layer with strong magnetostriction. Their probability depends on the history and number of repetitions of the field cycling, thus testifying the thermal-activation nature of the long-time relaxation of an antiferromagnetic order. These results provide evidence of spontaneous thermally activated switching of the antiferromagnetic order in NiO grains during magnetization reversal in ferromagnet/antiferromagnet (FM/AFM) heterostructures. The respective deformation modes are discussed in terms of the thermal fluctuation aftereffect in the Fulcomer and Charap model which predicts that irreversible breakdown of the original spin orientation can take place in some antiferromagnetic grains with disordered anisotropy axes during magnetization reversal of exchange-coupled FM/AFM structures. The spin reorientation in the saturated state may induce abrupt distortion of isolated metastable grains because of the NiO magnetostriction, leading to excitation of shock waves and formation of plate (or Lamb) waves.
Magnetic-field gradiometer based on ultracold collisions
Wasak, Tomasz; Jachymski, Krzysztof; Calarco, Tommaso; Negretti, Antonio
2018-05-01
We present a detailed analysis of the usefulness of ultracold atomic collisions for sensing the strength of an external magnetic field as well as its spatial gradient. The core idea of the sensor, which we recently proposed in Jachymski et al. [Phys. Rev. Lett. 120, 013401 (2018), 10.1103/PhysRevLett.120.013401], is to probe the transmission of the atoms through a set of quasi-one-dimensional waveguides that contain an impurity. Magnetic-field-dependent interactions between the incoming atoms and the impurity naturally lead to narrow resonances that can act as sensitive field probes since they strongly affect the transmission. We illustrate our findings with concrete examples of experimental relevance, demonstrating that for large atom fluences N a sensitivity of the order of 1 nT/√{N } for the field strength and 100 nT/(mm √{N }) for the gradient can be reached with our scheme.
Synthesis and Magnetic Properties of Maghemite (γ-Fe2O3 Short-Nanotubes
Directory of Open Access Journals (Sweden)
Xiao XH
2010-01-01
Full Text Available Abstract We report a rational synthesis of maghemite (γ-Fe2O3 short-nanotubes (SNTs by a convenient hydrothermal method and subsequent annealing process. The structure, shape, and magnetic properties of the SNTs were investigated. Room-temperature and low-temperature magnetic measurements show that the as-fabricated γ-Fe2O3 SNTs are ferromagnetic, and its coercivity is nonzero when the temperature above blocking temperature (TB. The hysteresis loop was operated to show that the magnetic properties of γ-Fe2O3 SNTs are strongly influenced by the morphology of the crystal. The unique magnetic behaviors were interpreted by the competition of the demagnetization energy of quasi-one-dimensional nanostructures and the magnetocrystalline anisotropy energy of particles in SNTs.
The spatially anisotropic triangular lattice antiferromagnet: Popov-Fedotov method
International Nuclear Information System (INIS)
Nga, Pham Thi Thanh; Trang, Phan Thu; Thang, Nguyen Toan
2017-01-01
We present an analysis of the antiferromagnetic Heisenberg model on an triangular lattice with spatially anisotropic J 1 - J 2 exchange interactions. We apply the Popov-Fedotov method based on introducing an imaginary valued chemical potential to enforce the auxiliary fermion constraint exactly. The staggered magnetization, magnon spectra, free energy are computed in one loop approximation and compared using two different constraints: exact and on average. In the limit of zero temperature the results are identical, whereas at higher temperature significant differences are found. The comparisons with the results obtained by other methods are discussed. (paper)
Quantum phase transitions of a disordered antiferromagnetic topological insulator
Baireuther, P.; Edge, J. M.; Fulga, I. C.; Beenakker, C. W. J.; Tworzydło, J.
2014-01-01
We study the effect of electrostatic disorder on the conductivity of a three-dimensional antiferromagnetic insulator (a stack of quantum anomalous Hall layers with staggered magnetization). The phase diagram contains regions where the increase of disorder first causes the appearance of surface conduction (via a topological phase transition), followed by the appearance of bulk conduction (via a metal-insulator transition). The conducting surface states are stabilized by an effective time-reversal symmetry that is broken locally by the disorder but restored on long length scales. A simple self-consistent Born approximation reliably locates the boundaries of this so-called "statistical" topological phase.
Anisotropic Magnetoresistance in Antiferromagnetic Sr_{2}IrO_{4}
Directory of Open Access Journals (Sweden)
C. Wang
2014-11-01
Full Text Available We report point-contact measurements of anisotropic magnetoresistance (AMR in a single crystal of antiferromagnetic Mott insulator Sr_{2}IrO_{4}. The point-contact technique is used here as a local probe of magnetotransport properties on the nanoscale. The measurements at liquid nitrogen temperature reveal negative magnetoresistances (up to 28% for modest magnetic fields (250 mT applied within the IrO_{2} a-b plane and electric currents flowing perpendicular to the plane. The angular dependence of magnetoresistance shows a crossover from fourfold to twofold symmetry in response to an increasing magnetic field with angular variations in resistance from 1% to 14%. We tentatively attribute the fourfold symmetry to the crystalline component of AMR and the field-induced transition to the effects of applied field on the canting of antiferromagnetic-coupled moments in Sr_{2}IrO_{4}. The observed AMR is very large compared to the crystalline AMRs in 3d transition metal alloys or oxides (0.1%–0.5% and can be associated with the large spin-orbit interactions in this 5d oxide while the transition provides evidence of correlations between electronic transport, magnetic order, and orbital states. The finding of this work opens an entirely new avenue to not only gain a new insight into physics associated with spin-orbit coupling but also to better harness the power of spintronics in a more technically favorable fashion.
Effects of interfacial frustration in ferromagnet/antiferromagnet bilayers
Urazhdin, Sergei; Ma, Tianyu
While the ferromagnet (F)/antiferromagnet (AF) bilayers have been extensively studied in the context of exchange bias, and more recently in the context of antiferromagnetic spintronics, the fundamental understanding of the nature of the magnetic state in this system is still a subject a debate. We will present measurements of magnetization aging in several F/AF systems based on AF=FeMn, CoO, and NiO, universally observed in all of these systems when AF layers are sufficiently thin. Quite generally, the aging curves are well-described by the power law with a small exponent. We show that the aging characteristics such as the dependence on temperature and the magnetic history are inconsistent with the Arrhenius activation, disproving the granular models of exchange bias. Furthermore, we show that the aging characteristics qualitatively change across the exchange bias blocking temperature, demonstrating that the latter is similar to the glass transition temperature, and is not simply of a characteristic activation temperature of the AF domains. We discuss the our findings in the context of frustration due to the random effective exchange field at the F/AF interface. supported by NSF DMR.
New concepts for molecular magnets
Pilawa, Bernd
1999-03-01
-paramagnetism and quasi one-dimensional magnets.
Dynamic rotor mode in antiferromagnetic nanoparticles
DEFF Research Database (Denmark)
Lefmann, Kim; Jacobsen, H.; Garde, J.
2015-01-01
We present experimental, numerical, and theoretical evidence for an unusual mode of antiferromagnetic dynamics in nanoparticles. Elastic neutron scattering experiments on 8-nm particles of hematite display a loss of diffraction intensity with temperature, the intensity vanishing around 150 K...
Magnetocaloric properties of a frustrated Blume-Capel antiferromagnet
Directory of Open Access Journals (Sweden)
Žukovič Milan
2014-07-01
Full Text Available Low-temperature magnetization processes and magnetocaloric properties of a geometrically frustrated spin-1 Blume-Capel model on a triangular lattice are studied by Monte Carlo simulations. The model is found to display qualitatively different behavior depending on the sign of the single-ion anisotropy D. For positive values of D we observe two magnetization plateaus, similar to the spin-1/2 Ising antiferromagnet, and negative isothermal entropy changes for any field intensity. For a range of small negative values of D there are four magnetization plateaus and the entropy changes can be either negative or positive, depending on the field. If D is negative but large in absolute value then the entropy changes are solely positive.
Magnon Spin Nernst Effect in Antiferromagnets
Zyuzin, Vladimir A.; Kovalev, Alexey A.
2016-11-01
We predict that a temperature gradient can induce a magnon-mediated spin Hall response in an antiferromagnet with nontrivial magnon Berry curvature. We develop a linear response theory which gives a general condition for a Hall current to be well defined, even when the thermal Hall response is forbidden by symmetry. We apply our theory to a honeycomb lattice antiferromagnet and discuss a role of magnon edge states in a finite geometry.
Magnon Spin Nernst Effect in Antiferromagnets.
Zyuzin, Vladimir A; Kovalev, Alexey A
2016-11-18
We predict that a temperature gradient can induce a magnon-mediated spin Hall response in an antiferromagnet with nontrivial magnon Berry curvature. We develop a linear response theory which gives a general condition for a Hall current to be well defined, even when the thermal Hall response is forbidden by symmetry. We apply our theory to a honeycomb lattice antiferromagnet and discuss a role of magnon edge states in a finite geometry.
Electronic structure of the antiferromagnetic phase of Sr2Co2O5
International Nuclear Information System (INIS)
Pardo, V.; Botta, P.M.; Baldomir, D.; Rivas, J.; Pineiro, A.; Calle, C. de la; Alonso, J.A.; Arias, J.E.
2008-01-01
Ab initio calculations analyze the properties of the G-type antiferromagnetic Sr 2 Co 2 O 5 as a high-spin system. The description of the electronic structure is given; all the Co atoms are in a high-spin state with a small unquenched orbital angular momentum. Thermal analysis on a polycrystalline sample shows a magnetic phase transition at high temperatures
Real-space imaging of non-collinear antiferromagnetic order with a single-spin magnetometer
Gross, I.; Akhtar, W.; Garcia, V.; Martínez, L. J.; Chouaieb, S.; Garcia, K.; Carrétéro, C.; Barthélémy, A.; Appel, P.; Maletinsky, P.; Kim, J.-V.; Chauleau, J. Y.; Jaouen, N.; Viret, M.; Bibes, M.; Fusil, S.; Jacques, V.
2017-09-01
Although ferromagnets have many applications, their large magnetization and the resulting energy cost for switching magnetic moments bring into question their suitability for reliable low-power spintronic devices. Non-collinear antiferromagnetic systems do not suffer from this problem, and often have extra functionalities: non-collinear spin order may break space-inversion symmetry and thus allow electric-field control of magnetism, or may produce emergent spin-orbit effects that enable efficient spin-charge interconversion. To harness these traits for next-generation spintronics, the nanoscale control and imaging capabilities that are now routine for ferromagnets must be developed for antiferromagnetic systems. Here, using a non-invasive, scanning single-spin magnetometer based on a nitrogen-vacancy defect in diamond, we demonstrate real-space visualization of non-collinear antiferromagnetic order in a magnetic thin film at room temperature. We image the spin cycloid of a multiferroic bismuth ferrite (BiFeO3) thin film and extract a period of about 70 nanometres, consistent with values determined by macroscopic diffraction. In addition, we take advantage of the magnetoelectric coupling present in BiFeO3 to manipulate the cycloid propagation direction by an electric field. Besides highlighting the potential of nitrogen-vacancy magnetometry for imaging complex antiferromagnetic orders at the nanoscale, these results demonstrate how BiFeO3 can be used in the design of reconfigurable nanoscale spin textures.
(Anti)-ferromagnetic coupling in Fe/Si multilayers from polarized neutron reflectomy
Fredrikze, H.; Graaf, van der A; Valkier, M.; Kohlhepp, J.T.; Broeder, den F.J.A.
1997-01-01
Polarized neutron reflectometry data on Fe/Si multilayers are interpreted using strongly depth-dependent magnetization in the Fe layers. This behaviour is ascribed to a depth-dependent mixture of ferromagnetic and anti-ferromagnetic coupled regions in the sample.
Antiferromagnetic CsCrF{sub 5} and canted antiferromagnetism in RbCrF{sub 5} and KCrF{sub 5}
Energy Technology Data Exchange (ETDEWEB)
Jagličić, Zvonko, E-mail: zvonko.jaglicic@imfm.si [University of Ljubljana, Faculty of Civil and Geodetic Engineering, and Institute of Mathematics, Physics and Mechanics, Jadranska 19, 1000 Ljubljana (Slovenia); Mazej, Zoran, E-mail: zoran.mazej@ijs.si [Department of Inorganic Chemistry and Technology, Jožef Stefan Institute, Jamova 39, 1000 Ljubljana (Slovenia)
2017-07-15
Highlights: • Cr(IV) ions are antiferromagnetically coupled within chains in ACrF{sub 5} (A = Cs, Rb, K). • Small structural difference causes huge difference in magnetic properties below 10 K. • Canted antiferromagnetism has been observed in RbCrF{sub 5} and KCrF{sub 5} at low temperature. - Abstract: In ACrF{sub 5} (A = Cs, Rb, K), Cr(IV) ions are coordinated by six fluoride ligands where the resulting CrF{sub 6} octahedra share cis vertexes to form infinite chains of ([Cr{sup IV}F{sub 5}]{sup −}){sub n}. The geometry of the latter in Cs compound differs from that in K and Rb compounds. The results of investigations of the magnetic behaviour of these compounds have shown that an antiferromagnetic superexchange interaction is present within the chains with J{sub Cs} = −10.2 cm{sup −1}, J{sub Rb} = −13.3 cm{sup −1}, and J{sub K} = −13.1 cm{sup −1}. Additional ferromagnetic-like long-range ordering has been observed in KCrF{sub 5} and RbCrF{sub 5} below 6 K which can be explained, in a correlation with their crystal structures, as canted antiferromagnetism.
Lee, Ki Hoon; Chung, Suk Bum; Park, Kisoo; Park, Je-Geun
2018-05-01
We investigated the topological property of magnon bands in the collinear magnetic orders of zigzag and stripe phases for the antiferromagnetic honeycomb lattice and identified Berry curvature and symmetry constraints on the magnon band structure. Different symmetries of both zigzag and stripe phases lead to different topological properties, in particular, the magnon bands of the stripe phase being disentangled with a finite Dzyaloshinskii-Moriya (DM) term with nonzero spin Chern number. This is corroborated by calculating the spin Nernst effect. Our study establishes the existence of a nontrivial magnon band topology for all observed collinear antiferromagnetic honeycomb lattices in the presence of the DM term.
Strain-Induced Ferromagnetism in Antiferromagnetic LuMnO3 Thin Films
White, J. S.; Bator, M.; Hu, Y.; Luetkens, H.; Stahn, J.; Capelli, S.; Das, S.; Döbeli, M.; Lippert, Th.; Malik, V. K.; Martynczuk, J.; Wokaun, A.; Kenzelmann, M.; Niedermayer, Ch.; Schneider, C. W.
2013-07-01
Single phase and strained LuMnO3 thin films are discovered to display coexisting ferromagnetic and antiferromagnetic orders. A large moment ferromagnetism (≈1μB), which is absent in bulk samples, is shown to display a magnetic moment distribution that is peaked at the highly strained substrate-film interface. We further show that the strain-induced ferromagnetism and the antiferromagnetic order are coupled via an exchange field, therefore demonstrating strained rare-earth manganite thin films as promising candidate systems for new multifunctional devices.
Nonmonotonic and anisotropic magnetoresistance effect in antiferromagnet CaMn2Bi2
Kawaguchi, N.; Urata, T.; Hatano, T.; Iida, K.; Ikuta, H.
2018-04-01
We found a large and unique magnetoresistance (MR) effect for CaMn2Bi2 . When the magnetic field was applied along the crystallographic c axis at low temperatures, the resistivity increased with the magnetic field and the MR ratio reached several hundred percent, but then it decreased with further increasing the applied field. In addition, the angle dependence measurement revealed a strong anisotropy. This compound is an antiferromagnetic semiconductor with a narrow band gap, and Mn atoms form a corrugated honeycomb lattice. Therefore, a frustration among the magnetic moments is expected, and we propose that our observations can be understood by a nonmonotonic modulation of magnetic fluctuation under the magnetic field.
Electrical control of antiferromagnetic metal up to 15 nm
Zhang, PengXiang; Yin, GuFan; Wang, YuYan; Cui, Bin; Pan, Feng; Song, Cheng
2016-08-01
Manipulation of antiferromagnetic (AFM) spins by electrical means is on great demand to develop the AFM spintronics with low power consumption. Here we report a reversible electrical control of antiferromagnetic moments of FeMn up to 15 nm, using an ionic liquid to exert a substantial electric-field effect. The manipulation is demonstrated by the modulation of exchange spring in [Co/Pt]/FeMn system, where AFM moments in FeMn pin the magnetization rotation of Co/Pt. By carrier injection or extraction, the magnetic anisotropy of the top layer in FeMn is modulated to influence the whole exchange spring and then passes its influence to the [Co/Pt]/FeMn interface, through a distance up to the length of exchange spring that fully screens electric field. Comparing FeMn to IrMn, despite the opposite dependence of exchange bias on gate voltages, the same correlation between carrier density and exchange spring stiffness is demonstrated. Besides the fundamental significance of modulating the spin structures in metallic AFM via all-electrical fashion, the present finding would advance the development of low-power-consumption AFM spintronics.
Fe-induced enhancement of antiferromagnetic spin correlations in Mn2-xFexBO4
Kazak, N. V.; Platunov, M. S.; Knyazev, Yu. V.; Moshkina, E. M.; Gavrilkin, S. Yu.; Bayukov, O. A.; Gorev, M. V.; Pogoreltsev, E. I.; Zeer, G. M.; Zharkov, S. M.; Ovchinnikov, S. G.
2018-04-01
Fe substitution effect on the magnetic behavior of Mn2-xFexBO4 (x = 0.3, 0.5, 0.7) warwickites has been investigated combining Mössbauer spectroscopy, dc magnetization, ac magnetic susceptibility, and heat capacity measurements. The Fe3+ ions distribution over two crystallographic nonequivalent sites is studied. The Fe introduction breaks a long-range antiferromagnetic order and leads to onset of spin-glass ground state. The antiferromagnetic short-range-order spin correlations persist up to temperatures well above TSG reflecting in increasing deviations from the Curie-Weiss law, the reduced effective magnetic moment and "missing" entropy. The results are interpreted in the terms of the progressive increase of the frustration effect and the formation of spin-correlated regions.
International Nuclear Information System (INIS)
Kavitha, L.; Saravanan, M.; Srividya, B.; Gopi, D.
2011-01-01
We investigate the nature of propagation of electromagnetic waves (EMWs) in an antiferromagnetic medium with Dzyaloshinsky-Moriya (DM) interaction environment. The interplay of bilinear and DM exchange spin coupling with the magnetic field component of the EMW has been studied by solving Maxwell's equations coupled with a nonlinear spin equation for the magnetization of the medium. We made a nonuniform expansion of the magnetization and magnetic field along the direction of propagation of EMW, in the framework of reductive perturbation method, and the dynamics of the system is found to be governed by a generalized derivative nonlinear Schroedinger (DNLS) equation. We employ the Jacobi-elliptic function method to solve the DNLS equation, and the electromagnetic wave propagation in an antiferromagnetic medium is governed by the breatherlike spatially and temporally coherent localized modes under the influence of DM interaction parameter.
Zero Modes and Global Antiferromagnetism in Strained Graphene
Directory of Open Access Journals (Sweden)
Bitan Roy
2014-05-01
Full Text Available A novel magnetic ground state is reported for the Hubbard Hamiltonian in strained graphene. When the chemical potential lies close to the Dirac point, the ground state exhibits locally both the Néel and ferromagnetic orders, even for weak Hubbard interaction. Whereas the Néel order parameter remains of the same sign in the entire system, the magnetization at the boundary takes the opposite sign from the bulk. The total magnetization vanishes this way, and the magnetic ground state is globally only an antiferromagnet. This peculiar ordering stems from the nature of the strain-induced single-particle zero-energy states, which have support on one sublattice of the honeycomb lattice in the bulk, and on the other sublattice near the boundary of a finite system. We support our claim with the self-consistent numerical calculation of the order parameters, as well as by the Monte Carlo simulations of the Hubbard model in both uniformly and nonuniformly strained honeycomb lattice. The present result is contrasted with the magnetic ground state of the same Hubbard model in the presence of a true magnetic field (and for vanishing Zeeman coupling, which is exclusively Néel ordered, with zero local magnetization everywhere in the system.
Wang, Kangkang; Smith, Arthur R
2012-11-14
Antiferromagnets play a key role in modern spintronic devices owing to their ability to modify the switching behavior of adjacent ferromagnets via the exchange bias effect. Consequently, detailed measurements of the spin structure at antiferromagnetic interfaces and surfaces are highly desirable, not only for advancing technologies but also for enabling new insights into the underlying physics. Here using spin-polarized scanning tunneling microscopy at room-temperature, we reveal in three-dimensions an orthogonal spin structure on antiferromagnetic compound nanopyramids. Contrary to expected uniaxial anisotropy based on bulk properties, the atomic terraces are found to have alternating in-plane and out-of-plane magnetic anisotropies. The observed layer-wise alternation in anisotropy could have strong influences on future nanoscale spintronic applications.
Quantum oscillations in antiferromagnetic CaFe2As2 on the brink of superconductivity
International Nuclear Information System (INIS)
Harrison, N; McDonald, R D; Mielke, C H; Bauer, E D; Ronning, F; Thompson, J D
2009-01-01
We report quantum oscillation measurements on CaFe 2 As 2 under strong magnetic fields-recently reported to become superconducting under pressures of as little as a kilobar. The largest observed carrier pocket occupies less than 0.05% of the paramagnetic Brillouin zone volume-consistent with Fermi surface reconstruction caused by antiferromagnetism. On comparing several alkaline earth AFe 2 As 2 antiferromagnets (with A = Ca, Sr and Ba), the dependences of the Fermi surface cross-sectional area F α and the effective mass m α * of the primary observed pocket on the antiferromagnetic/structural transition temperature T s are both found to be consistent with the case for quasiparticles in a conventional spin-density wave model. These findings suggest that the recently proposed strain-enhanced superconductivity in these materials occurs within a broadly conventional spin-density wave phase. (fast track communication)
Železný, J.
2017-01-10
One of the main obstacles that prevents practical applications of antiferromagnets is the difficulty of manipulating the magnetic order parameter. Recently, following the theoretical prediction [J. Železný, Phys. Rev. Lett. 113, 157201 (2014)]PRLTAO0031-900710.1103/PhysRevLett.113.157201, the electrical switching of magnetic moments in an antiferromagnet was demonstrated [P. Wadley, Science 351, 587 (2016)]SCIEAS0036-807510.1126/science.aab1031. The switching is due to the so-called spin-orbit torque, which has been extensively studied in ferromagnets. In this phenomena a nonequilibrium spin-polarization exchange coupled to the ordered local moments is induced by current, hence exerting a torque on the order parameter. Here we give a general systematic analysis of the symmetry of the spin-orbit torque in locally and globally noncentrosymmetric crystals. We study when the symmetry allows for a nonzero torque, when is the torque effective, and its dependence on the applied current direction and orientation of magnetic moments. For comparison, we consider both antiferromagnetic and ferromagnetic orders. In two representative model crystals we perform microscopic calculations of the spin-orbit torque to illustrate its symmetry properties and to highlight conditions under which the spin-orbit torque can be efficient for manipulating antiferromagnetic moments.
Železný , J.; Gao, H.; Manchon, Aurelien; Freimuth, Frank; Mokrousov, Yuriy; Zemen, J.; Mašek, J.; Sinova, Jairo; Jungwirth, T.
2017-01-01
One of the main obstacles that prevents practical applications of antiferromagnets is the difficulty of manipulating the magnetic order parameter. Recently, following the theoretical prediction [J. Železný, Phys. Rev. Lett. 113, 157201 (2014)]PRLTAO0031-900710.1103/PhysRevLett.113.157201, the electrical switching of magnetic moments in an antiferromagnet was demonstrated [P. Wadley, Science 351, 587 (2016)]SCIEAS0036-807510.1126/science.aab1031. The switching is due to the so-called spin-orbit torque, which has been extensively studied in ferromagnets. In this phenomena a nonequilibrium spin-polarization exchange coupled to the ordered local moments is induced by current, hence exerting a torque on the order parameter. Here we give a general systematic analysis of the symmetry of the spin-orbit torque in locally and globally noncentrosymmetric crystals. We study when the symmetry allows for a nonzero torque, when is the torque effective, and its dependence on the applied current direction and orientation of magnetic moments. For comparison, we consider both antiferromagnetic and ferromagnetic orders. In two representative model crystals we perform microscopic calculations of the spin-orbit torque to illustrate its symmetry properties and to highlight conditions under which the spin-orbit torque can be efficient for manipulating antiferromagnetic moments.
International Nuclear Information System (INIS)
Perez, J.F.; Pontin, L.F.; Segundo, J.A.B.
1985-01-01
Using a method proposed by van Hemmen the free energy of the Curie-Weiss version of the site-dilute antiferromagnetic Ising model is computed, in the presence of an uniform magnetic field. The solution displays an exact correspondence between this model and the Curie-Weiss version of the Ising model in the presence of a random magnetic field. The phase diagrams are discussed and a tricritical point is shown to exist. (Author) [pt
Adiabatic demagnetization of the antiferromagnetic spin-1/2 Heisenberg hexagonal cluster
International Nuclear Information System (INIS)
Deb, Moumita; Ghosh, Asim Kumar
2016-01-01
Exact analytic expressions of eigenvalues of the antiferromagnetic spin-1/2 Heisenberg hexagon in the presence of uniform magnetic field have been obtained. Magnetization process, nature of isentrops and properties of magneto caloric effect in terms of adiabatic demagnetization have been investigated. Theoretical results have been used to study the magneto caloric effect of the spin-1/2 Heisenberg hexagonal compound Cu_3WO_6.
Phase transition induced for external field in tree-dimensional isotropic Heisenberg antiferromagnet
Neto, Minos A.; Viana, J. Roberto; Salmon, Octavio D. R.; Filho, E. Bublitz; de Sousa, J. Ricardo
2017-01-01
In this paper, we report mean-field and effective-field renormalization group calculations on the isotropic Heisenberg antiferromagnetic model under a longitudinal magnetic field. As is already known, these methods, denoted by MFRG and EFRG, are based on the comparison of two clusters of different sizes, each of them trying to mimic certain Bravais lattice. Our attention has been on the obtantion of the critical frontier in the plane of temperature versus magnetic field, for the simple cubic ...
Antiferromagnetic ordering in GdRhIn{sub 5}
Energy Technology Data Exchange (ETDEWEB)
Latka, K.; Rams, M. [Marian Smoluchowski Inst. of Physics, Jagiellonian Univ., Krakow (Poland); Kmiec, R.; Pacyna, A.W. [Henryk Niewodniczanski Inst. of Nuclear Physics, Polish Academy of Sciences, Krakow (Poland); Zaremba, V.I. [Inorganic Chemistry Dept., Ivan Franko National Univ. of Lviv, Lviv (Ukraine); Inst. fuer Anorganische und Analytische Chemie, Westfaelische Wilhelms-Univ. Muenster (Germany); Poettgen, R. [Inst. fuer Anorganische und Analytische Chemie, Westfaelische Wilhelms-Univ. Muenster (Germany)
2004-09-01
A polycrystalline sample of tetragonal GdRhIn{sub 5} (HoCoGa{sub 5} type, space group P4/mmm) was obtained by induction melting of the elements in a glassy carbon crucible in a water-cooled sample chamber and subsequent annealing at 670 K. X-ray powder data yielded the cell parameters a = 460.65(7), c = 743.52(12) pm. The magnetic and electronic properties of GdRhIn{sub 5} have been studied by magnetic susceptibility, electrical resistivity, and {sup 155}Gd Moessbauer spectroscopic measurements. Antiferromagnetic ordering is detected at 41.0(2) K. The results are discussed using a simple molecular field approximation. (orig.)
Antiferromagnetic order in the ladder compound SrCu{sub 2}O{sub 3}: Cu-NMR/NQR measurements
Energy Technology Data Exchange (ETDEWEB)
Ohsugi, S.; Kitaoka, Y.; Azuma, M.; Fujishiro, Y.; Takano, M.
1999-12-01
The authors carried out the extensive Cu-nuclear magnetic and quadrupole resonance (NMR/NQR) experiments on the Zn(Ni)-doped ladder compound SrCu{sub 2}O{sub 3} (Sr123), Sr(Cu{sub 1{minus}x}M{sub x}){sub 2}O{sub 3} (M = Zn and Ni) with x {le} 0.02 and the La-doped Sr123, Sr{sub 1{minus}x}La{sub x}Cu{sub 2}O{sub 3} with {alpha} {le} 0.03. A spin-correlation length {xi}{sub s}/a (a: the lattice spacing between the Cu sites along the leg) of nonmagnetic impurity-induced staggered polarization (IISP) estimated from a quasi-one-dimensional (Q1D) IISP along the two legs in the 0.1--2% Zn-doped Sr123 was found to be independent of temperature (T) and scaled to an mean impurity distance D{sub AV} with the relation of {xi}{sub s}/a = 2.5 + D{sub AV}. The {xi}{sub s}/a's are much longer in x = 0.001 ({xi}{sub s}/a {approximately} 50) and 0.005 ({xi}{sub s}/a {approximately} 12) than an instantaneous spin-correlation length {xi}{sub 0}/a {approximately} 3--8 in Sr123. The formula of Neel T, T{sub N} (WC-Q1D) = J exp({minus}D{sub AV}/({xi}{sub s}/a)) (J = 2,000 K) based on the weakly interladder-coupled (WC) Q1D model explains the experimental T{sub N} values quantitatively.
Ground state configurations in antiferromagnetic ultrathin films with dipolar anisotropy
International Nuclear Information System (INIS)
León, H.
2013-01-01
The formalism developed in a previous work to calculate the dipolar energy in quasi-two-dimensional crystals with ferromagnetic order is now extended to collinear antiferromagnetic order. Numerical calculations of the dipolar energy are carried out for systems with tetragonally distorted fcc [001] structures, the case of NiO and MnO ultrathin film grown in non-magnetic substrates, where the magnetic phase is a consequence of superexchange and dipolar interactions. The employed approximation allows to demonstrate that dipolar coupling between atomic layers is responsible for the orientation of the magnetization when it differs from the one in a single layer. The ground state energy of a given NiO or MnO film is found to depend not only on the strain, but also on how much the interlayer separation and the 2D lattice constant are changed with respect to the ideal values corresponding to the non-distorted cubic structure. Nevertheless, it is shown that the orientation of the magnetization in the magnetic phase of any of these films is determined by the strain exclusively. A striped phase with the magnetization along the [112 ¯ ] direction appears as the ground state configuration of NiO and MnO ultrathin films. In films with equally oriented stripes along the layers this magnetic phase is twofold degenerate, while in films with multidomain layers it is eightfold degenerate. These results are not in contradiction with experimentally observed out-of-plane or in-plane magnetization of striped phases in NiO and MnO ultrathin films. - Highlights: ► Dipolar energy in collinear antiferromagnetic ultrathin films is calculated. ► Numerical results are presented for distorted fcc [001] structures. ► The lowest energy of a system depends on how the tetragonal distortion is achieved. ► A striped phase with magnetization in the [112 ¯ ] direction is the ground state. ► In multidomain NiO and MnO films it is eightfold degenerate.
Robust spin transfer torque in antiferromagnetic tunnel junctions
Saidaoui, Hamed Ben Mohamed; Waintal, Xavier; Manchon, Aurelien
2017-01-01
We theoretically study the current-induced spin torque in antiferromagnetic tunnel junctions, composed of two semi-infinite antiferromagnetic layers separated by a tunnel barrier, in both clean and disordered regimes. We find that the torque
Experimental validation of Villain's conjecture about magnetic ordering in quasi-1D helimagnets
Energy Technology Data Exchange (ETDEWEB)
Cinti, F., E-mail: fabio.cinti@fi.infn.i [CNISM and Department of Physics, University of Florence, 50019 Sesto Fiorentino (Italy); CNR-INFM S3 National Research Center, I-41100 Modena (Italy); Rettori, A. [CNISM and Department of Physics, University of Florence, 50019 Sesto Fiorentino (Italy); CNR-INFM S3 National Research Center, I-41100 Modena (Italy); Pini, M.G. [ISC-CNR, Via Madonna del Piano 10, I-50019 Sesto Fiorentino (Italy); Mariani, M.; Micotti, E. [Department of Physics A. Volta and CNR-INFM, University of Pavia, Via Bassi 6, I-27100 Pavia (Italy); Lascialfari, A. [Department of Physics A. Volta and CNR-INFM, University of Pavia, Via Bassi 6, I-27100 Pavia (Italy); Institute of General Physiology and Biological Chemistry, University of Milano, Via Trentacoste 2, I-20134 Milano (Italy); CNR-INFM S3 National Research Center, I-41100 Modena (Italy); Papinutto, N. [CIMeC, University of Trento, Via delle Regole, 101 38060 Mattarello (Italy); Department of Physics A. Volta and CNR-INFM, University of Pavia, Via Bassi 6, I-27100 Pavia (Italy); Amato, A. [Paul Scherrer Institute, CH-5232 Villingen PSI (Switzerland); Caneschi, A.; Gatteschi, D. [INSTM R.U. Firenze and Department of Chemistry, University of Florence, Via della Lastruccia 3, I-50019 Sesto Fiorentino (Italy); Affronte, M. [CNR-INFM S3 National Research Center, I-41100 Modena (Italy); Department of Physics, University of Modena and Reggio Emilia Via Campi 213/A, I-41100 Modena (Italy)
2010-05-15
Low-temperature magnetic susceptibility, zero-field muon spin resonance and specific heat measurements have been performed in the quasi-one-dimensional (1D) molecular helimagnetic compound Gd(hfac){sub 3}NITEt. The specific heat presents two anomalies at T{sub 0}=2.19(2)K and T{sub N}=1.88(2)K, while susceptibility and zero-field muon spin resonance show anomalies only at T{sub N}=1.88(2)K. The results suggest an experimental validation of Villain's conjecture of a two-step magnetic ordering in quasi-1D XY helimagnets: the paramagnetic phase and the helical spin solid phases are separated by a chiral spin liquid, where translational invariance is broken without violation of rotational invariance.
Experimental validation of Villain's conjecture about magnetic ordering in quasi-1D helimagnets
International Nuclear Information System (INIS)
Cinti, F.; Rettori, A.; Pini, M.G.; Mariani, M.; Micotti, E.; Lascialfari, A.; Papinutto, N.; Amato, A.; Caneschi, A.; Gatteschi, D.; Affronte, M.
2010-01-01
Low-temperature magnetic susceptibility, zero-field muon spin resonance and specific heat measurements have been performed in the quasi-one-dimensional (1D) molecular helimagnetic compound Gd(hfac) 3 NITEt. The specific heat presents two anomalies at T 0 =2.19(2)K and T N =1.88(2)K, while susceptibility and zero-field muon spin resonance show anomalies only at T N =1.88(2)K. The results suggest an experimental validation of Villain's conjecture of a two-step magnetic ordering in quasi-1D XY helimagnets: the paramagnetic phase and the helical spin solid phases are separated by a chiral spin liquid, where translational invariance is broken without violation of rotational invariance.
Bandstructure study of magnetic and orbital order in BaCoO3
International Nuclear Information System (INIS)
Pardo, V.; Blaha, P.; Iglesias, M.; Baldomir, D.; Schwarz, K.; Pereiro, M.; Botana, J.; Arias, J.E.
2005-01-01
Ab initio calculations were performed in the quasi-one-dimensional BaCoO 3 using the FP-APW+lo method as implemented in the WIEN2k package utilizing the LDA+U approach. Several magnetic configurations were studied, exploring different intra- and inter-chain couplings. The most stable configuration is the ferromagnetic low-spin state. The electronic structure of the Co 4+ ion (t 2g 5 ) has an orbital degree of freedom. When an 'alternating-orbital' ordering is allowed along the Co chains, the energy of the system is drastically reduced, whereas the magnetic order is a secondary effect. This orbital ordered state reproduces the experimentally found semiconducting behaviour, which is analysed studying the bandstructure of the material
Antiferromagnetic MnN layer on the MnGa(001) surface
Energy Technology Data Exchange (ETDEWEB)
Guerrero-Sánchez, J., E-mail: guerrero@cnyn.unam.mx; Takeuchi, Noboru
2016-12-30
Highlights: • A ferromagnetic Gallium terminated surface is stable before N incorporation. • After N incorporation, an antiferromagnetic MnN layer becomes stable in a wide range of chemical potential. • Spin density distribution shows an antiferromagnetic/ferromagnetic (MnN/MnGa) arrangement at the surface. - Abstract: Spin polarized first principles total energy calculations have been applied to study the stability and magnetic properties of the MnGa(001) surface and the formation of a topmost MnN layer with the deposit of nitrogen. Before nitrogen adsorption, surface formation energies show a stable gallium terminated ferromagnetic surface. After incorporation of nitrogen atoms, the antiferromagnetic manganese terminated surface becomes stable due to the formation of a MnN layer (Mn-N bonding at the surface). Spin density distribution shows a ferromagnetic/antiferromagnetic arrangement in the first surface layers. This thermodynamically stable structure may be exploited to growth MnGa/MnN magnetic heterostructures as well as to look for exchange biased systems.
Crystallographic and magnetic properties of (C6D11ND3)CuBr3 and (Zn1-xMnx)3As2
International Nuclear Information System (INIS)
Vries, G.C. de.
1989-08-01
The investigations described concern the crystallographic and magnetic properties of the quasi one-dimensional (1d) ferromagnetic system (C 6 D 11 ND 3 )CuBr 3 (or CHAB) and the II-V type diluted magnetic semiconductor (Zn 1 - x Mn x ) 3 As 2 (or ZMA). Both compounds have been studied with various neutron scattering techniques. The crystallographic properties of CHAB and ZMA have been investigated by neutron diffraction. These diffraction experiments were carried out at the High Flux Reactor (HFR) at Petten, Netherlands. For the investigation of the static and dynamic magnetic properties of CHAB neutron scattering experiments were performed in Petten as well as other European reactor institutes. These investigations comprise a study of the 3d long-rate order and the 1d correlations of the magnetic moments, and a study of the behaviour of the linear spin-wave excitations
Pure spin current manipulation in antiferromagnetically exchange coupled heterostructures
Avilés-Félix, L.; Butera, A.; González-Chávez, D. E.; Sommer, R. L.; Gómez, J. E.
2018-03-01
We present a model to describe the spin currents generated by ferromagnet/spacer/ferromagnet exchange coupled trilayer systems and heavy metal layers with strong spin-orbit coupling. By exploiting the magnitude of the exchange coupling (oscillatory RKKY-like coupling) and the spin-flop transition in the magnetization process, it has been possible to produce spin currents polarized in arbitrary directions. The spin-flop transition of the trilayer system originates pure spin currents whose polarization vector depends on the exchange field and the magnetization equilibrium angles. We also discuss a protocol to control the polarization sign of the pure spin current injected into the metallic layer by changing the initial conditions of magnetization of the ferromagnetic layers previously to the spin pumping and inverse spin Hall effect experiments. The small differences in the ferromagnetic layers lead to a change in the magnetization vector rotation that permits the control of the sign of the induced voltage components due to the inverse spin Hall effect. Our results can lead to important advances in hybrid spintronic devices with new functionalities, particularly, the ability to control microscopic parameters such as the polarization direction and the sign of the pure spin current through the variation of macroscopic parameters, such as the external magnetic field or the thickness of the spacer in antiferromagnetic exchange coupled systems.
Structure and dynamics of magnetic nanoparticles
DEFF Research Database (Denmark)
Clausen, K.N.; Bødker, F.; Hansen, M.F.
2000-01-01
In this paper we present X-ray and neutron diffraction data illustrating aspects of crystal and magnetic structures of ferromagnetic alpha-Fe and antiferromagnetic NiO nanoparticles, as well as inelastic neutron scattering studies of the magnetic fluctuations in NiO and in canted antiferromagnetic...
Hole pairing induced by antiferromagnetic spin fluctuations
International Nuclear Information System (INIS)
Su, Z.B.; Yu Lu; Dong, J.M.; Tosatti, E.
1987-08-01
The effective interaction induced by antiferromagnetic spin fluctuations is considered in the random phase approximation in the context of the recently discovered high T c oxide superconductors. This effective attraction favours a triplet pairing of holes. The implications of such pairing mechanism are discussed in connection with the current experimental observations. (author). 30 refs, 2 figs
Antiferromagnetism in chromium alloy single crystals
DEFF Research Database (Denmark)
Bjerrum Møller, Hans; Trego, A.L.; Mackintosh, A.R.
1965-01-01
The antiferromagnetism of single crystals of dilute alloys of V, Mn and Re in Cr has been studied at 95°K and 300°K by neutron diffraction. The addition of V causes the diffraction peaks to decrease in intensity and move away from (100), while Mn and Re cause them to increase and approach (100) s...
Metallic and antiferromagnetic fixed points from gravity
Paul, Chandrima
2018-06-01
We consider SU(2) × U(1) gauge theory coupled to matter field in adjoints and study RG group flow. We constructed Callan-Symanzik equation and subsequent β functions and study the fixed points. We find there are two fixed points, showing metallic and antiferromagnetic behavior. We have shown that metallic phase develops an instability if certain parametric conditions are satisfied.
Doped spin ladders under magnetic field
International Nuclear Information System (INIS)
Roux, G.
2007-07-01
This thesis deals with the physics of doped two-leg ladders which are a quasi one-dimensional and unconventional superconductor. We particularly focus on the properties under magnetic field. Models for strongly correlated electrons on ladders are studied using exact diagonalization and density-matrix renormalization group (DMRG). Results are also enlightened by using the bosonization technique. Taking into account a ring exchange it highlights the relation between the pairing of holes and the spin gap. Its influence on the dynamics of the magnetic fluctuations is also tackled. Afterwards, these excitations are probed by the magnetic field by coupling it to the spin degree of freedom of the electrons through Zeeman effect. We show the existence of doping-dependent magnetization plateaus and also the presence of an inhomogeneous superconducting phase (FFLO phase) associated with an exceeding of the Pauli limit. When a flux passes through the ladder, the magnetic field couples to the charge degree of freedom of the electrons via orbital effect. The diamagnetic response of the doped ladder probes the commensurate phases of the t-J model at low J/t. Algebraic transverse current fluctuations are also found once the field is turned on. Lastly, we report numerical evidences of a molecular superfluid phase in the 3/2-spin attractive Hubbard model: at a density low enough, bound states of four fermions, called quartets, acquire dominant superfluid fluctuations. The observed competition between the superfluid and density fluctuations is connected to the physics of doped ladders. (author)
Circular dichroism and Raman optical activity in antiferromagnetic transition metal fluorides
International Nuclear Information System (INIS)
Hoffman, K.R.; Lockwood, D.J.; Yen, W.M.
2005-01-01
The Raman optical activity (ROA) of magnons in rutile-structure antiferromagnetic FeF 2 (T N = 78 K) has been studied as a function of temperature and applied magnetic field. For exciting light incident along the c axis, ROA is observed for magnons but not for phonons. In zero field, a small splitting (0.09 cm -1 ) of the two acoustic-magnon branches is observed for the first time by inelastic light scattering. The splitting in applied magnetic field is found to reduce with increasing temperature in accordance with theory. No ROA was detected for two-magnon excitations. In optical absorption measurements performed over thirty years ago, a very small circular dichroism (CD) was observed in the magnon sidebands of other simple rutile antiferromagnetic fluorides (MnF 2 and CoF 2 ). The origin of this CD was not understood at the time. The Raman studies of the one-magnon Raman scattering in FeF 2 have demonstrated that in zero field the degeneracy of the antiferromagnetic magnon branches is lifted by a weak magnetic dipole-dipole interaction, as predicted by Pincus and Loudon and by White four decades ago. The source of the observed CD in the magnon sidebands can now be traced to this same magnetic-dipole induced splitting
Control and manipulation of antiferromagnetic skyrmions in racetrack
Xia, Haiyan; Jin, Chendong; Song, Chengkun; Wang, Jinshuai; Wang, Jianbo; Liu, Qingfang
2017-12-01
Controllable manipulations of magnetic skyrmions are essential for next-generation spintronic devices. Here, the duplication and merging of skyrmions, as well as logical AND and OR functions, are designed in antiferromagnetic (AFM) materials with a cusp or smooth Y-junction structures. The operational time are in the dozens of picoseconds, enabling ultrafast information processing. A key factor for the successful operation is the relatively complex Y-junction structures, where domain walls propagate through in a controlled manner, without significant risks of pinning, vanishing or unwanted depinning of existing domain walls, as well as the nucleation of new domain walls. The motions of a multi-bit, namely the motion of an AFM skyrmion-chain in racetrack, are also investigated. Those micromagnetic simulations may contribute to future AFM skyrmion-based spintronic devices, such as nanotrack memory, logic gates and other information processes.
Evolution of topological features in finite antiferromagnetic Heisenberg chains
International Nuclear Information System (INIS)
Chen Changfeng
2003-01-01
We examine the behavior of nonlocal topological order in finite antiferromagnetic Heisenberg chains using the density matrix renormalization group techniques. We find that chains with even and odd site parity show very different behavior in the topological string order parameter, reflecting interesting interplay of the intrinsic magnetic correlation and the topological term in the chains. Analysis of the calculated string order parameter as a function of the chain length and the topological angle indicates that S=1/2 and S=1 chains show special behavior while all S>1 chains have similar topological structure. This result supports an earlier conjecture on the classification of quantum spin chains based on an analysis of their phase diagrams. Implications of the topological behavior in finite quantum spin chains are discussed
Energy Technology Data Exchange (ETDEWEB)
Wu, R. [State Key Laboratory for Mesoscopic Physics, School of Physics, Peking University, Beijing 100871 (China); Department of Materials Science and Metallurgy, University of Cambridge, Cambridge CB3 0FS (United Kingdom); Yun, C.; Ding, S. L.; Wen, X.; Liu, S. Q.; Wang, C. S.; Han, J. Z.; Du, H. L. [State Key Laboratory for Mesoscopic Physics, School of Physics, Peking University, Beijing 100871 (China); Yang, J. B., E-mail: jbyang@pku.edu.cn [State Key Laboratory for Mesoscopic Physics, School of Physics, Peking University, Beijing 100871 (China); Collaborative Innovation Center of Quantum Matter, Beijing 100871 (China)
2016-08-07
The motion of antiferromagnetic interfacial spins is investigated through the temperature evolution of training effect in a Co/CoO film with in-plane biaxial anisotropy. Significant differences in the training effect and its temperature dependence are observed in the magnetic easy axis and hard axis (HA) and ascribed to the different motion modes of antiferromagnetic interfacial spins, the collective spin cluster rotation (CSR) and the single spin reversal (SSR), caused by different magnetization reversal modes of ferromagnetic layer. These motion modes of antiferromagnetic spins are successfully separated using a combination of an exponential function and a classic n{sup −1/2} function. A larger CSR to SSR ratio and a shorter lifetime of CSR found in the HA indicates that the domain rotation in the ferromagnetic layer tends to activate and accelerate a CSR mode in the antiferromagnetic spins.
International Nuclear Information System (INIS)
Wu, R.; Yun, C.; Ding, S. L.; Wen, X.; Liu, S. Q.; Wang, C. S.; Han, J. Z.; Du, H. L.; Yang, J. B.
2016-01-01
The motion of antiferromagnetic interfacial spins is investigated through the temperature evolution of training effect in a Co/CoO film with in-plane biaxial anisotropy. Significant differences in the training effect and its temperature dependence are observed in the magnetic easy axis and hard axis (HA) and ascribed to the different motion modes of antiferromagnetic interfacial spins, the collective spin cluster rotation (CSR) and the single spin reversal (SSR), caused by different magnetization reversal modes of ferromagnetic layer. These motion modes of antiferromagnetic spins are successfully separated using a combination of an exponential function and a classic n"−"1"/"2 function. A larger CSR to SSR ratio and a shorter lifetime of CSR found in the HA indicates that the domain rotation in the ferromagnetic layer tends to activate and accelerate a CSR mode in the antiferromagnetic spins.
Oxygen-induced immediate onset of the antiferromagnetic stacking in thin Cr films on Fe(001)
Energy Technology Data Exchange (ETDEWEB)
Berti, Giulia, E-mail: giulia.berti@polimi.it; Brambilla, Alberto; Calloni, Alberto; Bussetti, Gianlorenzo; Finazzi, Marco; Duò, Lamberto; Ciccacci, Franco [Dipartimento di Fisica, Politecnico di Milano, Piazza Leonardo da Vinci 32, I-20133 Milano (Italy)
2015-04-20
We investigated the magnetic coupling of ultra-thin Cr films grown at 600 K on a Fe(001)-p(1 × 1)O substrate by means of spin-polarized photoemission spectroscopy. Our findings show that the expected antiferromagnetic stacking of the magnetization in Cr(001) layers occurs right from the first atomic layer at the Cr/Fe interface. This is at variance with all previous observations in similar systems, prepared in oxygen-free conditions, which always reported on a delayed onset of the magnetic oscillations due to the occurrence of significant chemical alloying at the interface, which is substantially absent in our preparation.
Surface antiferromagnetism and incipient metal-insulator transition in strained manganite films
Cossu, Fabrizio; Colizzi, G.; Filippetti, A.; Fiorentini, Vincenzo; Schwingenschlö gl, Udo
2013-01-01
Using first-principles calculations, we show that the (001) surface of the ferromagnet La0.7Sr0.3MnO3 under an epitaxial compressive strain favors antiferromagnetic (AF) order in the surface layers, coexisting with ferromagnetic (FM) bulk order. Surface antiferromagnetism is accompanied by a very marked surface-related spectral pseudogap, signaling an incomplete metal-insulator transition at the surface. The different relaxation and rumpling of the MnO2 and LaO surface planes in the two competing magnetic phases cause distinct work-function changes, which are of potential diagnostic use. The AF phase is recognized as an extreme surface-assisted case of the combination of in-plane AF super-exchange and vertical FM double-exchange couplings that rules magnetism in manganites under in-plane compression.
Surface antiferromagnetism and incipient metal-insulator transition in strained manganite films
Cossu, Fabrizio
2013-06-21
Using first-principles calculations, we show that the (001) surface of the ferromagnet La0.7Sr0.3MnO3 under an epitaxial compressive strain favors antiferromagnetic (AF) order in the surface layers, coexisting with ferromagnetic (FM) bulk order. Surface antiferromagnetism is accompanied by a very marked surface-related spectral pseudogap, signaling an incomplete metal-insulator transition at the surface. The different relaxation and rumpling of the MnO2 and LaO surface planes in the two competing magnetic phases cause distinct work-function changes, which are of potential diagnostic use. The AF phase is recognized as an extreme surface-assisted case of the combination of in-plane AF super-exchange and vertical FM double-exchange couplings that rules magnetism in manganites under in-plane compression.
Dipolar Antiferromagnetism and Quantum Criticality in LiErF4
International Nuclear Information System (INIS)
Kraemer, Conradin; Nikseresht, Neda; Piatek, Julian; Tsyrulin, Nikolay; Piazza, Bastien; Kiefer, Klaus; Klemke, Bastian; Rosenbaum, Thomas; Aeppli, Gabriel; Gannarelli, Che; Prokes, Karel; Straessle, Thierry; Keller, Lukas; Zaharko, Oksana; Kraemer, Karl; Ronnow, Henrik
2012-01-01
Magnetism has been predicted to occur in systems in which dipolar interactions dominate exchange. We present neutron scattering, specific heat, and magnetic susceptibility data for LiErF 4 , establishing it as a model dipolar-coupled antiferromagnet with planar spin-anisotropy and a quantum phase transition in applied field H c# parallel# = 4.0 ± 0.1 kilo-oersteds. We discovered non-mean-field critical scaling for the classical phase transition at the antiferromagnetic transition temperature that is consistent with the two-dimensional XY/h 4 universality class; in accord with this, the quantum phase transition at H c exhibits three-dimensional classical behavior. The effective dimensional reduction may be a consequence of the intrinsic frustrated nature of the dipolar interaction, which strengthens the role of fluctuations.
'Aharonov-Bohm antiferromagnetism' and compensation points in the lattice of quantum rings
International Nuclear Information System (INIS)
Meleshenko, Peter A.; Klinskikh, Alexander F.
2011-01-01
We investigate the magnetic properties of the lattice of non-interacting quantum rings using the 2D rotator model. The exact analytic expressions for the free energy as well as for the magnetization and magnetic susceptibility are found and analyzed. It is shown that such a system can be considered as a system with antiferromagnetic-like properties. We have shown also that all observable quantities in this case (free energy, entropy, magnetization) are periodic functions of the magnetic flux through the ring's area (as well known, such a behavior is typical for the Aharonov-Bohm effect). For the lattice of quantum rings with two different geometric parameters we investigate the ordinary compensation points ('temperature compensation points', i.e. points at which the magnetization vanishes at fixed values of the magnetic field strength). It is shown that the positions of compensation points in the temperature scale are very sensitive to small changes in the magnetic field strength. - Highlights: → The lattice of quantum rings as a system with antiferromagnetic-like properties. → In considered system the 'temperature compensation points' take place. → The 'temperature compensation points' positions depend on the Aharonov-Bohm flux.
Energy Technology Data Exchange (ETDEWEB)
Gong, W. J.; Liu, W., E-mail: wliu@imr.ac.cn; Feng, J. N.; Zhang, Z. D. [Shenyang National Laboratory for Materials Science, Institute of Metal Research, Chinese Academy of Sciences, Shenyang 110016 (China); Kim, D. S.; Choi, C. J. [Functional Materials Division, Korea Institute of Materials Science, 531 Changwon- daero, Changwon 631-831 (Korea, Republic of)
2014-04-07
The effect of antiferromagnetic (AFM) layer on exchange bias (EB), training effect, and magnetotransport properties in ferromagnetic (FM) /AFM nanoscale antidot arrays and sheet films Ag(10 nm)/Co(8 nm)/NiO(t{sub NiO})/Ag(5 nm) at 10 K is studied. The AFM layer thickness dependence of the EB field shows a peak at t{sub NiO} = 2 nm that is explained by using the random field model. The misalignment of magnetic moments in the three-dimensional antidot arrays causes smaller decrease of EB field compared with that in the sheet films for training effect. The anomalous magnetotransport properties, in particular positive magnetoresistance (MR) for antidot arrays but negative MR for sheet films are found. The training effect and magnetotransport properties are strongly affected by the three-dimensional spin-alignment effects in the antidot arrays.
Anomalous Z2 antiferromagnetic topological phase in pressurized SmB6
Chang, Kai-Wei; Chen, Peng-Jen
2018-05-01
Antiferromagnetic materials, whose time-reversal symmetry is broken, can be classified into the Z2 topology if they respect some specific symmetry. Since the theoretical proposal, however, no materials have been found to host such Z2 antiferromagnetic topological (Z2-AFT ) phase to date. Here we demonstrate that the topological Kondo insulator SmB6 can be a Z2-AFT system when pressurized to undergo an antiferromagnetic phase transition. In addition to proposing the possible candidate for a Z2-AFT material, in this work we also illustrate the anomalous topological surface states of the Z2-AFT phase which have not been discussed before. Originating from the interplay between the topological properties and the antiferromagnetic surface magnetization, the topological surface states of the Z2-AFT phase behave differently as compared with those of a topological insulator. Besides, the Z2-AFT insulators are also found promising in the generation of tunable spin currents, which is an important application in spintronics.
Directory of Open Access Journals (Sweden)
Borovský Michal
2016-01-01
Full Text Available The population annealing algorithm is a novel approach to study systems with rough free-energy landscapes, such as spin glasses. It combines the power of simulated annealing, Boltzmann weighted differential reproduction and sequential Monte Carlo process to bring the population of replicas to the equilibrium even in the low-temperature region. Moreover, it provides a very good estimate of the free energy. The fact that population annealing algorithm is performed over a large number of replicas with many spin updates, makes it a good candidate for massive parallelism. We chose the GPU programming using a CUDA implementation to create a highly optimized simulation. It has been previously shown for the frustrated Ising antiferromagnet on the stacked triangular lattice with a ferromagnetic interlayer coupling, that standard Markov Chain Monte Carlo simulations fail to equilibrate at low temperatures due to the effect of kinetic freezing of the ferromagnetically ordered chains. We applied the population annealing to study the case with the isotropic intra- and interlayer antiferromagnetic coupling (J2/|J1| = −1. The reached ground states correspond to non-magnetic degenerate states, where chains are antiferromagnetically ordered, but there is no long-range ordering between them, which is analogical with Wannier phase of the 2D triangular Ising antiferromagnet.
Magnetic modes in superlattices
International Nuclear Information System (INIS)
Oliveira, F.A.
1990-04-01
A first discussion of reciprocal propagation of magnetic modes in a superlattice is presented. In the absence of an applied external magnetic field a superllatice made of alternate layers of the type antiferromagnetic-non-magnetic materials presents effects similar to those of phonons in a dielectric superlattice. (A.C.A.S.) [pt
Control of antiferromagnetic spin axis orientation in bilayer Fe/CuMnAs films
Czech Academy of Sciences Publication Activity Database
Wadley, P.; Edmonds, K. W.; Shahedkhah, M.R.; Campion, R. P.; Gallagher, B. L.; Železný, Jakub; Kuneš, Jan; Novák, Vít; Jungwirth, Tomáš; Saidl, Vít; Němec, P.; Maccherozzi, F.; Dhesi, S.S.
2017-01-01
Roč. 7, Sep (2017), 1-6, č. článku 11147. ISSN 2045-2322 R&D Projects: GA MŠk LM2015087; GA ČR GB14-37427G Institutional support: RVO:68378271 Keywords : antiferromagnetic spintronics * exchange coupling Subject RIV: BM - Solid Matter Physics ; Magnetism OBOR OECD: Condensed matter physics (including formerly solid state physics, supercond.) Impact factor: 4.259, year: 2016
Multiple-stable anisotropic magnetoresistance memory in antiferromagnetic MnTe
Czech Academy of Sciences Publication Activity Database
Kriegner, D.; Výborný, Karel; Olejník, Kamil; Reichlová, Helena; Novák, Vít; Martí, Xavier; Gazquez, J.; Saidl, V.; Němec, P.; Volobuev, V.V.; Springholz, G.; Holý, V.; Jungwirth, Tomáš
2016-01-01
Roč. 7, Jun (2016), 1-7, č. článku 11623. ISSN 2041-1723 R&D Projects: GA ČR GA15-13436S; GA MŠk(CZ) LM2011026; GA ČR GB14-37427G EU Projects: European Commission(XE) 268066 - 0MSPIN Institutional support: RVO:68378271 Keywords : antiferromagnets * spintronics * anisotropic magnetoresistance Subject RIV: BM - Solid Matter Physics ; Magnetism Impact factor: 12.124, year: 2016
High antiferromagnetic domain wall velocity induced by Néel spin-orbit torques
Czech Academy of Sciences Publication Activity Database
Gomonay, O.; Jungwirth, Tomáš; Sinova, Jairo
2016-01-01
Roč. 117, č. 1 (2016), 1-5, č. článku 017202. ISSN 0031-9007 R&D Projects: GA MŠk(CZ) LM2011026; GA ČR GB14-37427G EU Projects: European Commission(XE) 268066 - 0MSPIN Institutional support: RVO:68378271 Keywords : spintronics * domain walls * antiferromagnets Subject RIV: BM - Solid Matter Physics ; Magnetism Impact factor: 8.462, year: 2016
A critical scattering study of the helical antiferromagnets Ho and Dy
International Nuclear Information System (INIS)
Gaulin, B.D.; Hagen, M.; Child, H.R.
1988-01-01
We have measured the frequency integrated magnetic critical scattering of neutrons from paramagnetic Dy and Ho. Analysis of these data show the paramagnetic to helical antiferromagnetic phase transitions are characterized by the critical exponents ν = 0.57 +- 0.05 and γ = 1.05 = +- .07 for Dy and ν = 0.57 +- .04 and γ = 1.14 = +- .10 for Ho. 3 refs., 2 figs., 1 tab
Antiferromagnetic CuMnAs multi-level memory cell with microelectronic compatibility
Czech Academy of Sciences Publication Activity Database
Olejník, Kamil; Schuler, V.; Martí, Xavier; Novák, Vít; Kašpar, Zdeněk; Wadley, P.; Campion, R. P.; Edmonds, K. W.; Gallagher, B. L.; Garces, J.; Baumgartner, M.; Gambardella, P.; Jungwirth, Tomáš
2017-01-01
Roč. 8, May (2017), 1-7, č. článku 15434. ISSN 2041-1723 R&D Projects: GA MŠk LM2015087; GA ČR GB14-37427G EU Projects: European Commission(XE) 268066 - 0MSPIN Institutional support: RVO:68378271 Keywords : spintronics * antiferromagnets Subject RIV: BM - Solid Matter Physics ; Magnetism OBOR OECD: Condensed matter physics (including formerly solid state physics, supercond.) Impact factor: 12.124, year: 2016
Electrical measurement of antiferromagnetic moments in exchange-coupled IrMn/NiFe stacks
Czech Academy of Sciences Publication Activity Database
Martí, X.; Park, B.G.; Wunderlich, Joerg; Reichlová, Helena; Kurosaki, Y.; Yamada, M.; Yamamoto, H.; Nishide, A.; Hayakawa, J.; Takahashi, H.; Jungwirth, Tomáš
2012-01-01
Roč. 108, č. 1 (2012), , , "017201-1"-"017201-4" ISSN 0031-9007 EU Projects: European Commission(XE) 268066 - 0MSPIN Grant - others:AV ČR(CZ) AP0801 Program:Akademická prémie - Praemium Academiae Institutional research plan: CEZ:AV0Z10100521 Keywords : tunneling magnetoresistance * antiferromagnetic spintronics * exchange bias Subject RIV: BM - Solid Matter Physics ; Magnetism Impact factor: 7.943, year: 2012
Relativistic Néel-order fields induced by electrical current in antiferromagnets
Czech Academy of Sciences Publication Activity Database
Železný, Jakub; Gao, H.; Výborný, Karel; Zemen, Jan; Mašek, Jan; Manchon, A.; Wunderlich, Joerg; Sinova, Jairo; Jungwirth, Tomáš
2014-01-01
Roč. 113, č. 15 (2014), , "157201-1"-"157201-5" ISSN 0031-9007 R&D Projects: GA MŠk(CZ) LM2011026; GA ČR GB14-37427G EU Projects: European Commission(XE) 268066 - 0MSPIN Institutional support: RVO:68378271 Keywords : spintronics * antiferromagnets * current induced switching Subject RIV: BM - Solid Matter Physics ; Magnetism Impact factor: 7.512, year: 2014
Theory of antiferromagnetic pairing in cuprate superconductors
International Nuclear Information System (INIS)
Plakida, N.M.
2006-01-01
A review of the antiferromagnetic exchange and spin-fluctuation pairing theory in the cuprate superconductors is given. We briefly discuss a phenomenological approach and a theory in the limit of weak Coulomb correlations. A microscopic theory in the strong correlation limit is presented in more detail. In particular, results of our recently developed theory for the effective p-d Hubbard model and the reduced t-J model are given. We have proved that retardation effects for the antiferromagnetic exchange interaction are unimportant that results in pairing of all charge carriers in the conduction band and high Tc proportional to the Fermi energy. The spin-fluctuation interaction caused by kinematic interaction gives an additional contribution to the d-wave pairing. Dependence of Tc on the hole concentration and the lattice constant (or pressure) and an oxygen isotope shift are discussed
High field magnetoresistance and de Haas-van Alphen effect in antiferromagnetic PrB6 and NdB6
International Nuclear Information System (INIS)
Onuki, Y.; Umezawa, A.; Kwok, W.K.; Crabtree, G.W.; Nishihara, M.; Yamazaki, T.; Omi, T.; Komatsubara, T.
1987-08-01
The transport properties and the de Haas-van Alphen (dHvA) effect have been measured for antiferromagnetic PrB 6 and NdB 6 . The number of conduction electrons is approximately one per unit cell. The magnetoresistance shows the existence of open orbits implying a multiply connected Fermi surface. The angular dependence of the magnetoresistance is roughly similar to that of the reference material, LaB 6 . The dHvA data in PrB 6 shows both paramagnetic and antiferromagnetic Fermi surfaces. The antiferromagnetic Fermi surface arises from new magnetic Brillouin zone boundaries and antiferromagnetic gaps introduced by the magnetic order, and the paramagnetic Fermi surface from magnetic breakdown through the small antiferromagnetic gaps in high field. Hybridization between the conduction electrons and the f electrons has been observed through the cyclotron masses, which in PrB 6 are three times larger than the corresponding masses of LaB 6 . In NdB 6 only the antiferromagnetic Fermi surface, quite different from those of LaB 6 and PrB 6 , has been observed. 26 refs., 10 figs., 3 tabs
Entanglement in a Dimerized Antiferromagnetic Heisenberg Chain
Hao, Xiang; Zhu, Shiqun
2008-01-01
The entanglement properties in an antiferromagnetic dimerized Heisenberg spin-1/2 chain are investigated. The entanglement gap, which is the difference between the ground-state energy and the minimal energy that any separable state can attain, is calculated to detect the entanglement. It is found that the entanglement gap can be increased by varying the alternation parameter. Through thermal energy, the witness of the entanglement can determine a characteristic temperature below that an entan...
International Nuclear Information System (INIS)
Javed, Qurat-ul-ain; Feng-Ping Wang; Rafique, M. Yasir; Toufiq, Arbab Mohammad; Iqbal, M. Zubair
2012-01-01
We have reported new magnetic and optical properties of Mn 2 O 3 nanostructures. The nanostructures have been synthesized by the hydrothermal method combined with the adjustment of pH values in the reaction system. The particular characteristics of the nanostructures have been analyzed by employing X-Ray diffraction (XRD), scanning electron microscopy (SEM), energy dispersive X-ray (EDX) analysis, transmission electron microscopy (TEM), high resolution transmission electron microscopy (HRTEM), Raman spectroscopy (RS), UV—visible spectroscopy, and the vibrating sample magnetometer (VSM). Structural investigation manifests that the synthesized Mn 2 O 3 nanostructures are orthorhombic crystal. Magnetic investigation indicates that the Mn 2 O 3 nanostructures are antiferromagnetic and the antiferromagnetic transition temperature is at T N = 83 K. Furthermore, the Mn 2 O 3 nanostructures possess canted antiferromagnetic order below the Neel temperature due to spin frustration, resulting in hysteresis with large coercivity (1580 Oe) and remnant magnetization (1.52 emu/g). The UV—visible spectrophotometry was used to determine the transmittance behaviour of Mn 2 O 3 nanostructures. A direct optical band gap of 1.2 eV was acquired by using the Davis—Mott model. The UV—visible spectrum indicates that the absorption is prominent in the visible region, and transparency is more than 80% in the UV region
Antiferromagnetism and its origin in iron-based superconductors (Review Article)
International Nuclear Information System (INIS)
Ding, Ming-Cui; Zhang, Yu-Zhong; Lin, Hai-Qing
2014-01-01
In iron-based superconductors, unravelling the origin of the antiferromagnetism is a crucial step towards understanding the high-T c superconductivity as it is widely believed that the magnetic fluctuations play important roles in the formation of the Cooper pairs. Therefore, in this paper, we will briefly review experimental results related to the antiferromagnetic state in iron-based superconductors and focus on a review of the theoretical investigations which show applicability of the itinerant scenario to the observed antiferromagnetism and corresponding phase transitions in various families of the iron-based superconductors. A proposal of coupling between frustrated and un frustrated bands for understanding the reduced magnetic moment typically observed in iron pnictides is also reviewed. While all the above theoretical investigations do not rule out a possible existence of localized electrons in iron-based superconductors, these results strongly indicate a close relation between itinerant electrons and the magnetically ordered state and point out the importance of taking into account the orbital degrees of freedom.
Hugdal, Henning G.; Rex, Stefan; Nogueira, Flavio S.; Sudbø, Asle
2018-05-01
We study the effective interactions between Dirac fermions on the surface of a three-dimensional topological insulator due to the proximity coupling to the magnetic fluctuations in a ferromagnetic or antiferromagnetic insulator. Our results show that the magnetic fluctuations can mediate attractive interactions between Dirac fermions of both Amperean and BCS types. In the ferromagnetic case, we find pairing between fermions with parallel momenta, so-called Amperean pairing, whenever the effective Lagrangian for the magnetic fluctuations does not contain a quadratic term. The pairing interaction also increases with increasing Fermi momentum and is in agreement with previous studies in the limit of high chemical potential. If a quadratic term is present, the pairing is instead of BCS type above a certain chemical potential. In the antiferromagnetic case, BCS pairing occurs when the ferromagnetic coupling between magnons on the same sublattice exceeds the antiferromagnetic coupling between magnons on different sublattices. Outside this region in parameter space, we again find that Amperean pairing is realized.
Model calculation of thermal conductivity in antiferromagnets
Energy Technology Data Exchange (ETDEWEB)
Mikhail, I.F.I., E-mail: ifi_mikhail@hotmail.com; Ismail, I.M.M.; Ameen, M.
2015-11-01
A theoretical study is given of thermal conductivity in antiferromagnetic materials. The study has the advantage that the three-phonon interactions as well as the magnon phonon interactions have been represented by model operators that preserve the important properties of the exact collision operators. A new expression for thermal conductivity has been derived that involves the same terms obtained in our previous work in addition to two new terms. These two terms represent the conservation and quasi-conservation of wavevector that occur in the three-phonon Normal and Umklapp processes respectively. They gave appreciable contributions to the thermal conductivity and have led to an excellent quantitative agreement with the experimental measurements of the antiferromagnet FeCl{sub 2}. - Highlights: • The Boltzmann equations of phonons and magnons in antiferromagnets have been studied. • Model operators have been used to represent the magnon–phonon and three-phonon interactions. • The models possess the same important properties as the exact operators. • A new expression for the thermal conductivity has been derived. • The results showed a good quantitative agreement with the experimental data of FeCl{sub 2}.
Enhanced room temperature ferromagnetism in antiferromagnetic NiO nanoparticles
Energy Technology Data Exchange (ETDEWEB)
Ravikumar, Patta; Kisan, Bhagaban; Perumal, A., E-mail: perumal@iitg.ernet.in [Department of Physics, Indian institute of Technology Guwahati, Guwahati 781 039 (India)
2015-08-15
We report systematic investigations of structural, vibrational, resonance and magnetic properties of nanoscale NiO powders prepared by ball milling process under different milling speeds for 30 hours of milling. Structural properties revealed that both pure NiO and as-milled NiO powders exhibit face centered cubic structure, but average crystallite size decreases to around 11 nm along with significant increase in strain with increasing milling speed. Vibrational properties show the enhancement in the intensity of one-phonon longitudinal optical (LO) band and disappearance of two-magnon band due to size reduction. In addition, two-phonon LO band exhibits red shift due to size-induced phonon confinement effect and surface relaxation. Pure NiO powder exhibit antiferromagnetic nature, which transforms into induced ferromagnetic after size reduction. The average magnetization at room temperature increases with decreasing the crystallite size and a maximum moment of 0.016 μ{sub B}/f.u. at 12 kOe applied field and coercivity of 170 Oe were obtained for 30 hours milled NiO powders at 600 rotation per minute milling speed. The change in the magnetic properties is also supported by the vibrational properties. Thermomagnetization measurements at high temperature reveal a well-defined magnetic phase transition at high temperature (T{sub C}) around 780 K due to induced ferromagnetic phase. Electron paramagnetic resonance (EPR) studies reveal a good agreement between the EPR results and magnetic properties. The observed results are described on the basis of crystallite size variation, defect density, large strain, oxidation/reduction of Ni and interaction between uncompensated surfaces and particle core with lattice expansion. The obtained results suggest that nanoscale NiO powders with high T{sub C} and moderate magnetic moment at room temperature with cubic structure would be useful to expedite for spintronic devices.
Enhanced room temperature ferromagnetism in antiferromagnetic NiO nanoparticles
Directory of Open Access Journals (Sweden)
Patta Ravikumar
2015-08-01
Full Text Available We report systematic investigations of structural, vibrational, resonance and magnetic properties of nanoscale NiO powders prepared by ball milling process under different milling speeds for 30 hours of milling. Structural properties revealed that both pure NiO and as-milled NiO powders exhibit face centered cubic structure, but average crystallite size decreases to around 11 nm along with significant increase in strain with increasing milling speed. Vibrational properties show the enhancement in the intensity of one-phonon longitudinal optical (LO band and disappearance of two-magnon band due to size reduction. In addition, two-phonon LO band exhibits red shift due to size-induced phonon confinement effect and surface relaxation. Pure NiO powder exhibit antiferromagnetic nature, which transforms into induced ferromagnetic after size reduction. The average magnetization at room temperature increases with decreasing the crystallite size and a maximum moment of 0.016 μB/f.u. at 12 kOe applied field and coercivity of 170 Oe were obtained for 30 hours milled NiO powders at 600 rotation per minute milling speed. The change in the magnetic properties is also supported by the vibrational properties. Thermomagnetization measurements at high temperature reveal a well-defined magnetic phase transition at high temperature (TC around 780 K due to induced ferromagnetic phase. Electron paramagnetic resonance (EPR studies reveal a good agreement between the EPR results and magnetic properties. The observed results are described on the basis of crystallite size variation, defect density, large strain, oxidation/reduction of Ni and interaction between uncompensated surfaces and particle core with lattice expansion. The obtained results suggest that nanoscale NiO powders with high TC and moderate magnetic moment at room temperature with cubic structure would be useful to expedite for spintronic devices.
Magnetoelectric antiferromagnets as platforms for the manipulation of solitons
Zarzuela, Ricardo; Kim, Se Kwon; Tserkovnyak, Yaroslav
2018-01-01
We study the magnetic dynamics of magnetoelectric antiferromagnetic thin films, where an unconventional boundary ferromagnetism coexists with the bulk Néel phase below the Néel temperature. The spin exchange between the two order parameters yields an effective low-energy theory that is formally equivalent to that of a ferrimagnet. Dynamics of domain walls and skyrmions are analyzed within the collective-variable approach, from which we conclude that they behave as massive particles moving in a viscous medium subjected to a gyrotropic force. We find that the film thickness can be used as a control parameter for the motion of these solitons. In this regard, it is shown that an external magnetic field can drive the dynamics of domain walls, whose terminal velocity is tunable with the sample thickness. Furthermore, the classification of the skyrmion dynamics is sensitive to the spatial modulation of the sample thickness, which can be easily engineered with the present (thin-film) deposition techniques. Current-driven spin transfer can trigger drifting orbits of skyrmions, which can be utilized as racetracks for these magnetic textures.
Antiferromagnetic ordering in the plumbide EuPdPb
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Heletta, Lukas; Klenner, Steffen; Block, Theresa; Poettgen, Rainer [Muenster Univ. (Germany). Inst. fuer Anorganische und Analytische Chemie
2017-07-01
The plumbide EuPdPb was synthesized in polycrystalline form by reaction of the elements in a sealed niobium ampoule in a muffle furnace. The structure was refined from single-crystal X-ray diffractometer data: TiNiSi type, Pnma, a = 752.4(2), b = 476.0(2), c = 826.8(2) pm, wR2 = 0.0485, 704 F{sup 2} values and 20 variables. The europium atoms are coordinated by two tilted and puckered Pd{sub 3}Pb{sub 3} hexagons (280-289 pm Pd-Pb) with pronounced Eu-Pd bonding (312-339 pm). Temperature-dependent magnetic susceptibility measurements show Curie-Weiss behaviour and an experimental magnetic moment of 7.35(1) μB per Eu atom. EuPdPb orders antiferromagnetically at T{sub N} = 13.8(5) K and shows a metamagnetic transition at a critical field of 15 kOe. {sup 151}Eu Moessbauer spectra confirm divalent europium (δ = -10.04(1) mm s{sup -1}) and show full magnetic hyperfine field splitting (B{sub hf} = 21.1(1) T) at 6 K.
Charge dynamics of the antiferromagnetically ordered Mott insulator
International Nuclear Information System (INIS)
Han, Xing-Jie; Li, Xin; Chen, Jing; Liao, Hai-Jun; Xiang, Tao; Liu, Yu; Liu, Zhi-Yuan; Xie, Zhi-Yuan; Normand, B
2016-01-01
We introduce a slave-fermion formulation in which to study the charge dynamics of the half-filled Hubbard model on the square lattice. In this description, the charge degrees of freedom are represented by fermionic holons and doublons and the Mott-insulating characteristics of the ground state are the consequence of holon–doublon bound-state formation. The bosonic spin degrees of freedom are described by the antiferromagnetic Heisenberg model, yielding long-ranged (Néel) magnetic order at zero temperature. Within this framework and in the self-consistent Born approximation, we perform systematic calculations of the average double occupancy, the electronic density of states, the spectral function and the optical conductivity. Qualitatively, our method reproduces the lower and upper Hubbard bands, the spectral-weight transfer into a coherent quasiparticle band at their lower edges and the renormalisation of the Mott gap, which is associated with holon–doublon binding, due to the interactions of both quasiparticle species with the magnons. The zeros of the Green function at the chemical potential give the Luttinger volume, the poles of the self-energy reflect the underlying quasiparticle dispersion with a spin-renormalised hopping parameter and the optical gap is directly related to the Mott gap. Quantitatively, the square-lattice Hubbard model is one of the best-characterised problems in correlated condensed matter and many numerical calculations, all with different strengths and weaknesses, exist with which to benchmark our approach. From the semi-quantitative accuracy of our results for all but the weakest interaction strengths, we conclude that a self-consistent treatment of the spin-fluctuation effects on the charge degrees of freedom captures all the essential physics of the antiferromagnetic Mott–Hubbard insulator. We remark in addition that an analytical approximation with these properties serves a vital function in developing a full understanding of
Charge dynamics of the antiferromagnetically ordered Mott insulator
Han, Xing-Jie; Liu, Yu; Liu, Zhi-Yuan; Li, Xin; Chen, Jing; Liao, Hai-Jun; Xie, Zhi-Yuan; Normand, B.; Xiang, Tao
2016-10-01
We introduce a slave-fermion formulation in which to study the charge dynamics of the half-filled Hubbard model on the square lattice. In this description, the charge degrees of freedom are represented by fermionic holons and doublons and the Mott-insulating characteristics of the ground state are the consequence of holon-doublon bound-state formation. The bosonic spin degrees of freedom are described by the antiferromagnetic Heisenberg model, yielding long-ranged (Néel) magnetic order at zero temperature. Within this framework and in the self-consistent Born approximation, we perform systematic calculations of the average double occupancy, the electronic density of states, the spectral function and the optical conductivity. Qualitatively, our method reproduces the lower and upper Hubbard bands, the spectral-weight transfer into a coherent quasiparticle band at their lower edges and the renormalisation of the Mott gap, which is associated with holon-doublon binding, due to the interactions of both quasiparticle species with the magnons. The zeros of the Green function at the chemical potential give the Luttinger volume, the poles of the self-energy reflect the underlying quasiparticle dispersion with a spin-renormalised hopping parameter and the optical gap is directly related to the Mott gap. Quantitatively, the square-lattice Hubbard model is one of the best-characterised problems in correlated condensed matter and many numerical calculations, all with different strengths and weaknesses, exist with which to benchmark our approach. From the semi-quantitative accuracy of our results for all but the weakest interaction strengths, we conclude that a self-consistent treatment of the spin-fluctuation effects on the charge degrees of freedom captures all the essential physics of the antiferromagnetic Mott-Hubbard insulator. We remark in addition that an analytical approximation with these properties serves a vital function in developing a full understanding of the
Antiferromagnetic coupling of TbPc2 molecules to ultrathin Ni and Co films
Directory of Open Access Journals (Sweden)
David Klar
2013-05-01
Full Text Available The magnetic and electronic properties of single-molecule magnets are studied by X-ray absorption spectroscopy and X-ray magnetic circular dichroism. We study the magnetic coupling of ultrathin Co and Ni films that are epitaxially grown onto a Cu(100 substrate, to an in situ deposited submonolayer of TbPc2 molecules. Because of the element specificity of the X-ray absorption spectroscopy we are able to individually determine the field dependence of the magnetization of the Tb ions and the Ni or Co film. On both substrates the TbPc2 molecules couple antiferromagnetically to the ferromagnetic films, which is possibly due to a superexchange interaction via the phthalocyanine ligand that contacts the magnetic surface.
International Nuclear Information System (INIS)
Oubelkacem, A.; El Aouad, N.; Bentaleb, M.; Laaboudi, B.; Saber, M.
2004-01-01
Using the effective field theory with a probability distribution technique that accounts for the self-spin correlation functions, the magnetic properties of the diluted Ising superlattice consisting of two ferromagnetic materials A and B, with L a layers of diluted spins S a =((1)/(2)) and L b layers of diluted spins S b =1 with antiferromagnetic interface coupling are examined. For fixed values of the reduced exchange interactions and the concentration c of magnetic atoms, the phase diagrams, the two sublattice magnetizations and the total magnetization for the superlattice with the same spin S a =S b =((1)/(2)) and for S a =((1)/(2)), S b =1 are studied as a function of the temperature. We find a number of characteristic phenomena. In particular, the effect of the concentration c of magnetic atoms, the interlayer coupling and the layer thickness on both the compensation temperature and the magnetization profiles are clarified
Robust spin transfer torque in antiferromagnetic tunnel junctions
Saidaoui, Hamed Ben Mohamed
2017-04-18
We theoretically study the current-induced spin torque in antiferromagnetic tunnel junctions, composed of two semi-infinite antiferromagnetic layers separated by a tunnel barrier, in both clean and disordered regimes. We find that the torque enabling electrical manipulation of the Néel antiferromagnetic order parameter is out of plane, ∼n×p, while the torque competing with the antiferromagnetic exchange is in plane, ∼n×(p×n). Here, p and n are the Néel order parameter direction of the reference and free layers, respectively. Their bias dependence shows behavior similar to that in ferromagnetic tunnel junctions, the in-plane torque being mostly linear in bias, while the out-of-plane torque is quadratic. Most importantly, we find that the spin transfer torque in antiferromagnetic tunnel junctions is much more robust against disorder than that in antiferromagnetic metallic spin valves due to the tunneling nature of spin transport.
Siebbeles, L.D.A.; Movaghar, B.
2000-01-01
Using Monte Carlo simulations we calculate the frequency dependence of the diffusive mobility of a group of carriers on a short one-dimensional chain. We allow the carriers to interact with each other through weakly screened long-range Coulomb potentials. We consider both doped systems with discrete
Jackson, Howard; Badada, Bekele; Shi, Teng; Smith, Leigh; Zheng, Changlin; Etheridge, Joanne; Jiang, Nian; Tan, Hoe; Jagadish, Channupati
We explore the nature of exciton localization in single GaAs/AlGaAs nanowire quantum well tube (QWT) devices using photocurrent (PC) spectroscopy combined with simultaneous photoluminescence (PL) and photoluminescence excitation (PLE) measurements. Excitons confined to GaAs quantum well tubes of 8 and 4 nm widths embedded into an AlGaAs barrier are seen to ionize at high bias. Spectroscopic signatures of the ground and excited states confined to the QWT seen in PL, PLE and PC data are consistent with simple numerical calculations. The demonstration of good electrical contact with the QWTs enables the study of Stark effect shifts in the sharp emission lines of excitons localized to quantum dot-like states within the QWT. Atomic resolution cross-sectional TEM measurements, an analysis of the temperature dependence of PL and time-resolved PL as well as the quantum confined Stark effect of these dots provide insights into the nature of the exciton localization in these nanostructures. We acknowledge the financial support of NSF DMR 1507844, DMR 151373 and ECCS 1509706 and the Australian Research Council.
International Nuclear Information System (INIS)
Girardeau, M. D.; Minguzzi, A.
2010-01-01
In their Comment Giraud and Combescot (GC) [Phys. Rev. A 82, 037603 (2010)] point out that the contribution to the impurity-boson distribution function ρ bi (x-y) of a term we dropped is not negligible, rather than being negligible in the thermodynamic limit as we had conjectured. We now agree with them, but our results for ρ bi are highly accurate for large impurity-boson mass ratio m i /m, for all values of x-y and boson-impurity coupling constant.
Energy Technology Data Exchange (ETDEWEB)
Liu, K M; Juang, C H; Hsu, S Y [Department of Electrophysics, National Chiao Tung University, Hsinchu 30010, Taiwan (China); Umansky, V, E-mail: syhsu@mail.nctu.edu.t [Braun Center for Submicron Research, Weizmann Institute of Science, Rehovot 76100 (Israel)
2010-10-06
We have studied the linear conductance and source-drain bias spectroscopies of clean and disordered quantum wires (QWs) against thermal cycling and lateral shifting, which change the impurity configuration. Conductance quantization and the zero bias anomaly (ZBA) are robust in clean QWs. In contrast, disordered QWs show complexities in the ways of conductance resonance, peak splitting and trace crossing in source-drain bias spectroscopies. The experimental results and theoretical predictions are in congruence. Moreover, the resonant state arising from the impurities results in either a single peak or double-splitting peaks in the spectroscopies from the detailed impurity configurations. The resonant splitting peaks are found to influence the ZBA, indicating that a clean QW is crucial for investigating the intrinsic characteristics of the ZBA of QWs.
International Nuclear Information System (INIS)
Liu, K M; Juang, C H; Hsu, S Y; Umansky, V
2010-01-01
We have studied the linear conductance and source-drain bias spectroscopies of clean and disordered quantum wires (QWs) against thermal cycling and lateral shifting, which change the impurity configuration. Conductance quantization and the zero bias anomaly (ZBA) are robust in clean QWs. In contrast, disordered QWs show complexities in the ways of conductance resonance, peak splitting and trace crossing in source-drain bias spectroscopies. The experimental results and theoretical predictions are in congruence. Moreover, the resonant state arising from the impurities results in either a single peak or double-splitting peaks in the spectroscopies from the detailed impurity configurations. The resonant splitting peaks are found to influence the ZBA, indicating that a clean QW is crucial for investigating the intrinsic characteristics of the ZBA of QWs.
Exact ground and excited states of an antiferromagnetic quantum spin model
International Nuclear Information System (INIS)
Bose, I.
1989-08-01
A quasi-one-dimensional spin model which consists of a chain of octahedra of spins has been suggested for which a certain parameter regime of the Hamiltonian, the ground state, can be written down exactly. The ground state is highly degenerate and can be other than a singlet. Also, several excited states can be constructed exactly. The ground state is a local RVB state for which resonance is confined to rings of spins. Some exact numerical results for an octahedron of spins have also been reported. (author). 16 refs, 2 figs, 1 tab
International Nuclear Information System (INIS)
Baumann, J.; Seyboth, D.; Sontheimer, F.
1975-01-01
With the aim of determining the magnetic anisotropy of the lattice of antiferromagnetic FeGe 2 , Moessbauer spectra were measured on polycrystalline samples at 4.2 K in an external magnetic field varying from 0 to 80 kOe and at room temperature. A model was considered of a uniaxial antiferromagnet with one easy direction; assuming a random distribution of the symmetry axes of unit cells with respect to the external magnetic field, the ratio of the areas of the first two Moessbauer lines and the whole spectra were computed for several magnetic fields. A comparison with the measured spectra showed that the model could explain the measured values and the spectra at least qualitatively; to bring about a quantitative agreement, the authors modified the model by assuming a preferred orientation of the symmetry axes with regard to the external field. (A.K.)
Turov, Evgenii A.; Shavrov, Vladimir G.
1983-07-01
This review of some aspects of the magnetoacoustics of ferro- and antiferromagnetic materials has been written in connection with the 25th anniversary of the rise of this field of physics of magnetic phenomena. Primary attention is paid to relatively new problems that have not been reflected in the existing monographs and reviews. The topic is a group of linear magnetoacoustic effects that manifest spontaneous symmetry breaking caused by magnetic ordering in a system of two coupled fields: the magnetization field M (r) and the deformation field uij(r). To some extent these effects are analogous to the Higgs effect in the theory of elementary particles (the Higgs mechanism of the origin of the mass of a particle) or the Meissner effect in the theory of superconductivity. A direct analog of the stated effects is the so-called magnetoelastic gap in the magnon spectrum, while an analog of an accompanying effect is the softening of the quasiacoustic modes interacting with it (up to the vanishing of the corresponding dynamic elastic moduli). However, a characteristic feature of such effects in crystalline (anisotropic) magnetic materials is that they are manifested mainly near points of magnetic (spin-reorientation) phase transitions. This review treats the coupled magnetoelastic waves in ferro- and antiferromagnetic materials of different types that show phase transitions with respect to temperature, magnetic field, or pressure.
Photoemission electron microscopy for the study of ferromagnetic and antiferromagnetic materials
International Nuclear Information System (INIS)
Anders, Simone; Scholl, Andreas; Nolting, Frithjof; Padmore, Howard A.; Luening, Jan; Stoehr, Joachim; Scheinfein, Michael
2000-01-01
Photoemission electron microscopy (PEEM) is a full field imaging technique where x-ray exited electrons are used to form an image of the sample surface as a function of the x-ray photon energy and polarization. Contrast in PEEM can be due to a number of mechanisms including topographical, work function, elemental, chemical, polarization, x-ray magnetic circular and linear dichroism contrast. This wide range of contrast mechanisms together with the surface sensitivity and high spatial resolution make PEEM a very useful tool for the study of magnetic materials. PEEM-II is a new microscope installed at the bending magnet beamline 7.3.1.1 of the Advanced Light Source. In the present paper we describe the design and features of PEEM-II, and show results of our recent studies. Using PEEM and its elemental specificity, it is possible to investigate the various layers in magnetic multilayer structures independently. The experiments described here include the investigation of the switching behavior of magnetic multilayer structures that are of interest for magnetic RAM applications. The study of antiferromagnetic surfaces and thin films are of great importance for devices based on the effect of exchange bias. To date, studies at high-spatial-resolution of exchange bias systems has been difficult because of the lack of appropriate investigation methods. Here we demonstrate how PEEM has been used to image antiferromagnetic structure on surfaces with high spatial resolution
Czech Academy of Sciences Publication Activity Database
Kratochvílová, M.; Prokleška, J.; Uhlířová, K.; Tkáč, V.; Dušek, Michal; Sechovský, V.; Custers, J.
2015-01-01
Roč. 5, Oct (2015), s. 15904 ISSN 2045-2322 R&D Projects: GA ČR(CZ) GAP204/11/0809 Institutional support: RVO:68378271 Keywords : crystal structure * magnetic transition * heavy fermion compounds * antiferromagnetism Subject RIV: BM - Solid Matter Physics ; Magnetism Impact factor: 5.228, year: 2015
Frustrated antiferromagnets at high fields: Bose-Einstein condensation in degenerate spectra
International Nuclear Information System (INIS)
Jackeli, G.; Zhitomirsky, M.E.
2004-01-01
Quantum phase transition at the saturation field is studied for a class of frustrated quantum antiferromagnets. The considered models include (i) the J 1 -J 2 frustrated square-lattice antiferromagnet with J 2 =(1/2)J 1 and (ii) the nearest-neighbor Heisenberg antiferromagnet on a face centered cubic lattice. In the fully saturated phase the magnon spectra for the two models have lines of degenerate minima. Transition into a partially magnetized state is treated via a mapping to a dilute gas of hard-core bosons and by complementary spin-wave calculations. Momentum dependence of the exact four-point boson vertex removes the degeneracy of the single-particle excitation spectra and selects the ordering wave vectors at (π,π) and (π,0,0) for the two models. We predict a unique form for the magnetization curve ΔM=S-M≅μ (d-1)/2 (logμ) (d-1) , where μ is a distance from the quantum critical point
NMR studies of incommensurate quantum antiferromagnetic state of LiCuVO{sub 4}
Energy Technology Data Exchange (ETDEWEB)
Smith, R. [NHMFL, Florida State University, 1800 E P.Dirac Dr., Tallahassee FL 32310 (United States); Reyes, A.P. [NHMFL, Florida State University, 1800 E P.Dirac Dr., Tallahassee FL 32310 (United States); Ashey, R. [NHMFL, Florida State University, 1800 E P.Dirac Dr., Tallahassee FL 32310 (United States); Caldwell, T. [NHMFL, Los Alamos, NM 87545 (United States); Prokofiev, A. [Goethe University, 60054 Frankfurt (Germany); Assmus, W. [Goethe University, 60054 Frankfurt (Germany); Teitel' baum, G. [E.K.Zavoiskii Institute for Technical Physics of the RAS, Sibirskii Trakt 10/7, Kazan 420029 (Russian Federation)]. E-mail: grteit@kfti.knc.ru
2006-05-01
Our {sup 51}V NMR measurements in the LiCuVO{sub 4} single crystal reveal that the classical quadrupole split signal transforms upon lowering temperature to the single line with the shape typical for the systems undergoing the phase transition to the incommensurate magnetic state. The angular dependence of such a lineshape together with the anomalies of the {sup 51}V nuclear spin relaxation rates make it possible to conclude that the low-temperature magnetic order corresponds to the antiferromagnetic state with the incommensurate modulation along the b-axis of the crystal.
NMR studies of incommensurate quantum antiferromagnetic state of LiCuVO 4
Smith, R.; Reyes, A. P.; Ashey, R.; Caldwell, T.; Prokofiev, A.; Assmus, W.; Teitel'baum, G.
2006-05-01
Our 51V NMR measurements in the LiCuVO 4 single crystal reveal that the classical quadrupole split signal transforms upon lowering temperature to the single line with the shape typical for the systems undergoing the phase transition to the incommensurate magnetic state. The angular dependence of such a lineshape together with the anomalies of the 51V nuclear spin relaxation rates make it possible to conclude that the low-temperature magnetic order corresponds to the antiferromagnetic state with the incommensurate modulation along the b-axis of the crystal.
Large exchange-dominated domain wall velocities in antiferromagnetically coupled nanowires
Kuteifan, Majd; Lubarda, M. V.; Fu, S.; Chang, R.; Escobar, M. A.; Mangin, S.; Fullerton, E. E.; Lomakin, V.
2016-04-01
Magnetic nanowires supporting field- and current-driven domain wall motion are envisioned for methods of information storage and processing. A major obstacle for their practical use is the domain-wall velocity, which is traditionally limited for low fields and currents due to the Walker breakdown occurring when the driving component reaches a critical threshold value. We show through numerical and analytical modeling that the Walker breakdown limit can be extended or completely eliminated in antiferromagnetically coupled magnetic nanowires. These coupled nanowires allow for large domain-wall velocities driven by field and/or current as compared to conventional nanowires.
Dimensional dependence of exchange interactions at high magnetic fields
International Nuclear Information System (INIS)
Zehnder, U.; Kuhn-Heinrich, B.; Ossau, W.; Waag, A.; Landwehr, G.; Cheng, H.H.; Nicholas, R.J.
1996-01-01
We studied the contribution of the breaking of the antiferromagnetically coupled spin clusters to the total magnetization in thin (CdMn)Te layers as a function of the layer thickness by reflectivity spectroscopy in magnetic fields up to 45 T. The experimental results show that the contribution of the breaking of antiferromagnetically coupled spin clusters is reduced by decreasing layer thickness. (author)
International Nuclear Information System (INIS)
Jiang Jianjun; Liu Yongjun; Tang Fei; Yang Cuihong
2011-01-01
We investigated the properties of the spin-1/2 ferromagnetic-antiferromagnetic-antiferromagnetic alternating Heisenberg chain using the spin-wave theory. The spin-wave excitation spectra, the sublattice magnetizations and the local bond energies of the model are calculated to be compared with the corresponding properties of the mixed spin (1, 1/2) chain for a range of α. The results demonstrate that all the properties show similar behaviours in the small α limit, so the properties of the mixed spin (1, 1/2) chain can be described using the spin-1/2 ferromagnetic-antiferromagnetic-antiferromagnetic alternating Heisenberg chain. -- Research Highlights: →The spin-wave excitation spectra, the sublattice magnetizations and the local bond energies of the spin-1/2 ferromagnetic-antiferromagnetic-antiferromagnetic alternating Heisenberg chain are calculated. →In the small α limit, the properties of the mixed spin (1,1/2) chain can be described using the spin-1/2 ferromagnetic-antiferromagnetic-antiferromagnetic alternating Heisenberg chain. →The spin-1/2 ferromagnetic-antiferromagnetic-antiferromagnetic alternating Heisenberg chain may be of interest for some real quasi-one-dimensional molecular magnetic materials.
Antiferromagnetic spin fluctuations in the heavy-fermion superconductor Ce2PdIn8
Tran, V. H.; Hillier, A. D.; Adroja, D. T.; Kaczorowski, D.
2012-09-01
Inelastic neutron scattering and muon spin relaxation/rotation (μSR) measurements were performed on the heavy-fermion superconductor Ce2PdIn8. The observed scaling of the imaginary part of the dynamical susceptibility χ''Tα∝f(ℏω/kBT) with α=3/2 revealed a non-Fermi liquid character of the normal state, being due to critical antiferromagnetic fluctuations near a T=0 quantum phase transition. The longitudinal-field μSR measurements indicated that superconductivity and antiferromagnetic spin fluctuations coexist in Ce2PdIn8 on a microscopic scale. The observed power-law temperature dependence of the magnetic penetration depth λ∝T3/2, deduced from the transverse-field μSR data, strongly confirms an unconventional superconductivity in this compound.
International Nuclear Information System (INIS)
Magalhaes, S.G.; Zimmer, F.M.; Kipper, C.J.; Calegari, E.J.
2007-01-01
The competition among spin glass (SG), antiferromagnetism (AF) and local pairing superconductivity (PAIR) is studied in a two-sublattice fermionic Ising SG model with a local BCS pairing interaction in the presence of a transverse magnetic field Γ. The spins in different sublattices interact with Gaussian random couplings with an antiferromagnetic mean. The problem is formulated in a Grassmann path integral formalism. The static ansatz and the replica symmetry are used to obtain the half-filling thermodynamic potential. The results are shown in phase diagrams that exhibit a complex transition line separating the PAIR phase from the others. This line is second order at high temperature which ends in a tricritical point. The presence of Γ affects deeply the transition lines
Tunnelling anisotropic magnetoresistance due to antiferromagnetic CoO tunnel barriers
Wang, K.; Sanderink, J. G. M.; Bolhuis, T.; van der Wiel, W. G.; de Jong, M. P.
2015-01-01
A new approach in spintronics is based on spin-polarized charge transport phenomena governed by antiferromagnetic (AFM) materials. Recent studies have demonstrated the feasibility of this approach for AFM metals and semiconductors. We report tunneling anisotropic magnetoresistance (TAMR) due to the rotation of antiferromagnetic moments of an insulating CoO layer, incorporated into a tunnel junction consisting of sapphire(substrate)/fcc-Co/CoO/AlOx/Al. The ferromagnetic Co layer is exchange coupled to the AFM CoO layer and drives rotation of the AFM moments in an external magnetic field. The results may help pave the way towards the development of spintronic devices based on AFM insulators. PMID:26486931
Generation of Elliptically Polarized Terahertz Waves from Antiferromagnetic Sandwiched Structure.
Zhou, Sheng; Zhang, Qiang; Fu, Shu-Fang; Wang, Xuan-Zhang; Song, Yu-Ling; Wang, Xiang-Guang; Qu, Xiu-Rong
2018-04-01
The generation of elliptically polarized electromagnetic wave of an antiferromagnetic (AF)/dielectric sandwiched structure in the terahertz range is studied. The frequency and external magnetic field can change the AF optical response, resulting in the generation of elliptical polarization. An especially useful geometry with high levels of the generation of elliptical polarization is found in the case where an incident electromagnetic wave perpendicularly illuminates the sandwiched structure, the AF anisotropy axis is vertical to the wave-vector and the external magnetic field is pointed along the wave-vector. In numerical calculations, the AF layer is FeF2 and the dielectric layers are ZnF2. Although the effect originates from the AF layer, it can be also influenced by the sandwiched structure. We found that the ZnF2/FeF2/ZnF2 structure possesses optimal rotation of the principal axis and ellipticity, which can reach up to about thrice that of a single FeF2 layer.
Spintronic materials and devices based on antiferromagnetic metals
Directory of Open Access Journals (Sweden)
Y.Y. Wang
2017-04-01
Full Text Available In this paper, we review our recent experimental developments on antiferromagnet (AFM spintronics mainly comprising Mn-based noncollinear AFM metals. IrMn-based tunnel junctions and Hall devices have been investigated to explore the manipulation of AFM moments by magnetic fields, ferromagnetic materials and electric fields. Room-temperature tunneling anisotropic magnetoresistance based on IrMn as well as FeMn has been successfully achieved, and electrical control of the AFM exchange spring is realized by adopting ionic liquid. In addition, promising spin-orbit effects in AFM as well as spin transfer via AFM spin waves reported by different groups have also been reviewed, indicating that the AFM can serve as an efficient spin current source. To explore the crucial role of AFM acting as efficient generators, transmitters, and detectors of spin currents is an emerging topic in the field of magnetism today. AFM metals are now ready to join the rapidly developing fields of basic and applied spintronics, enriching this area of solid-state physics and microelectronics.
Lowest excited-state impurity binding energy in InGaN/GaN parabolic QWW: magnetic field effect
International Nuclear Information System (INIS)
Haddou El Ghazi; Anouar Jorio; Izeddine Zorkani
2013-01-01
In this paper, we have investigated the magnetic field effect on the lowest excited-state binding energy of hydrogenic shallow-donor impurity in wurtzite (In,Ga)N/GaN parabolic transversal-section quantum-well wire (PQWW) using the finite-difference method within the quasi-one-dimensional effective potential model. The calculations are performed within the framework of the effective mass approximation. A cylindrical QWW effective radius is taken into account to describe the lateral confinement strength. The numerical results show that: (i) the probability density is the largest on a circularity whose radius is the effective radius and (ii) the lowest excited-state binding energy is the largest when an impurity is located on this circularity while it starts to decrease as the impurity is away from the circularity. (author)
International Nuclear Information System (INIS)
Oubelkacem, A.; El Aouad, N.; Benaboud, A.; Saber, M.
2004-01-01
Using the effective field theory with a probability distribution technique that accounts for the self-spin correlation functions, the magnetic properties of the Ising superlattice consisting of two ferromagnetic materials A and B, with L a layers of diluted spins S a =((1)/(2)) and L b layers of diluted spins S b =1 in an applied transverse field Ω with antiferromagnetic interface coupling are examined. For fixed values of the reduced exchange interactions and the concentration c of magnetic atoms, the phase diagrams and the total magnetization for the superlattice are studied as a function of the transverse field and the temperature. We find a number of characteristic phenomena. In particular, the effect of the concentration c of magnetic atoms, the interlayer coupling and the transverse field on both the compensation temperature and the magnetization profiles are clarified. Some of them may be related to the experimental works of rare-earth (RE)/transition metal (TM) multilayer films
Solitary Magnons in the S =5/2 Antiferromagnet CaFe2O4
Stock, C.; Rodriguez, E. E.; Lee, N.; Green, M. A.; Demmel, F.; Ewings, R. A.; Fouquet, P.; Laver, M.; Niedermayer, Ch.; Su, Y.; Nemkovski, K.; Rodriguez-Rivera, J. A.; Cheong, S.-W.
2016-07-01
CaFe2O4 is a S =5/2 anisotropic antiferromagnet based upon zig-zag chains having two competing magnetic structures, denoted as the A (↑↑↓↓) and B (↑↓↑↓) phases, which differ by the c -axis stacking of ferromagnetic stripes. We apply neutron scattering to demonstrate that the competing A and B phase order parameters result in magnetic antiphase boundaries along c which freeze on the time scale of ˜1 ns at the onset of magnetic order at 200 K. Using high resolution neutron spectroscopy, we find quantized spin wave levels and measure 9 such excitations localized in regions ˜1 - 2 c -axis lattice constants in size. We discuss these in the context of solitary magnons predicted to exist in anisotropic systems. The magnetic anisotropy affords both competing A +B orders as well as localization of spin excitations in a classical magnet.
Thermoelectric properties of layered antiferromagnetic CuCrSe2
International Nuclear Information System (INIS)
Tewari, Girish C.; Tripathi, T.S.; Yamauchi, Hisao; Karppinen, Maarit
2014-01-01
Here we study thermoelectric and magnetic properties of CuCrSe 2 samples sintered at various temperatures. Structural analysis with XRD shows an order-disorder transition for Cr atoms when the sintering temperature is increased above 1273 K. Metal-like electrical resistivity and anomalously large Seebeck coefficient are found about room temperature. Analysis of electrical conductivity and Seebeck coefficient of the partially-disordered phase suggests hopping conduction of charge carriers. For both the ordered and disordered phases magnetic susceptibility follows Curie–Weiss temperature dependence at high temperatures above 150 K and shows an antiferromagnetic transition around 55 K. For the disordered phase, the effective magnetic moment is determined at 3.62 μ B ; this low value in comparison to the spin only value for Cr 3+ of 3.89 μ B indicates spin fluctuations in the paramagnetic state. The thermal conductivity in these phases is low and dominated by the lattice contribution. Values for the thermoelectric figure of merit (ZT) at room temperature are estimated to be 0.17 and 0.05 for the ordered and disordered phases, respectively. - Highlights: • Thermoelectric and magnetic properties of CuCrSe 2 samples are investigated. • The properties strongly depend on the degree of order of chromium atoms. • The degree of order is controlled by the sintering temperature. • Room-temperature figure of merit is estimated at 0.17 for the ordered phase. • For the disordered phase the figure of merit is lower
NMR studies of the helical antiferromagnetic compound EuCo2P2
Higa, N.; Ding, Q.-P.; Kubota, F.; Uehara, H.; Yogi, M.; Furukawa, Y.; Sangeetha, N. S.; Johnston, D. C.; Nakamura, A.; Hedo, M.; Nakama, T.; Ōnuki, Y.
2018-05-01
In EuCo2P2, 4f electron spins of Eu2+ ions order antiferromagnetically below a Néel temperature TN = 66.5 K . The magnetic structure below TN was reported to be helical with the helix axis along the c-axis from the neutron diffraction study. We report the results of 153Eu, 59Co and 31P nuclear magnetic resonance (NMR) measurements on EuCo2P2 using a single crystal and a powdered sample. In the antiferromagnetic (AFM) state, we succeeded in observing 153Eu, 59Co and 31P NMR spectra in zero magnetic field. The sharp 153Eu zero field NMR (ZF NMR) lines indicate homogeneous Eu ordered moment. The 59Co and 31P ZF NMR spectra showed an asymmetric spectral shape, indicating a distribution of the internal magnetic induction at each nuclear position. The AFM propagation vector k characterizing the helical AFM state can be determined from the internal magnetic induction at Co site. We have determined the model-independent value of the AFM propagation vector k distributed from (0, 0, 0.86)2π/c to (0, 0, 0.73)2π/c, where c is the lattice parameter.
Magnetic fluctuations in heavy-fermion metals
DEFF Research Database (Denmark)
Mason, T.E.; Petersen, T.; Aeppli, G.
1995-01-01
Elastic and inelastic neutron scattering have been used to study the antiferromagnetic ordering and magnetic excitations of the U heavy-fermion superconductors UPd2Al3 and URu2Si2 above and below T-N. While both materials exhibit the coexistence of superconductivity and antiferromagnetic order......, the nature of the antiferromagnetic order and magnetic fluctuations is qualitatively quite different. UPd2Al3 resembles a rare earth magnetic system with coupling of the 4f electrons to the conduction electrons manifested in a broadening of otherwise conventional spin wave excitations. This is in marked...