Polarization transfer in inelastic scattering

International Nuclear Information System (INIS)

Moss, J.M.

1980-01-01

Polarization transfer experiments are now feasible for inelastic scattering experiments on complex nuclei. Experiments thus far have dealt with the spin-flip probability; this observable is sensitive to the action of spin-spin and tensor forces in inelastic scattering. Spin-flip probabilities at E approx. 40 MeV in isoscalar transitions in 12 C(12.71 MeV) and 15 O(8.89 MeV) show considerable deviation from DWBA-shell model predictions; this deviation indicates evidence for more complex reaction mechanisms. Experiments at intermediate energies will soon be possible and will yield data of much higher precision than is possible at lower (E < 100 MeV) energies. These experiments hold exciting promise in such areas as nuclear critical opalescence. 7 figures, 1 table

Spin transfer matrix formulation and snake resonances for polarized proton beams

International Nuclear Information System (INIS)

Tepikian, S.

1986-01-01

The polarization of a spin polarized proton beam in a circular accelerator is described by a spin transfer matrix. Using this method, they investigate three problems: (1) the crossing of multiple spin resonances, (2) resonance jumping and (3) an accelerator with Siberian snakes. When crossing two (or more) spin resonances, there are no analytic solutions available. However, they can obtain analytic expressions if the two spin resonances are well separated (nonoverlapping) or very close together (overlapping). Between these two extremes they resort to numerical solution of the spin equations. Resonance jumping can be studied using the tools developed for analyzing the cross of multiple spin resonances. These theoretical results compare favorably with experimental results obtained from the AGS at Brookhaven. For large accelerators, resonance jumping becomes impractical and other methods such as Siberian snakes must be used to keep the beam spin polarized. An accelerator with Siberian snakes and isolated spin resonances can be described with a spin transfer matrix. From this, they find a new type of spin depolarizing resonance, called snake resonances

Polarized Radiative Transfer in Fluctuating Stochastic Media

International Nuclear Information System (INIS)

Sallah, M.; Degheidy, A.R.; Selim, M.M.

2009-01-01

The problem of polarized radiative transfer in a planar cluttered atmospheric medium (like cloudy atmosphere) is proposed. The solution is presented for an arbitrary absorption and scattering cross sections. The extinction function of the medium is assumed to be a continuous random function of position, with fluctuations about the mean taken as Gaussian distributed. The joint probability distribution function of these Gaussian random variables is used to calculate the ensemble-averaged quantities, such as reflectivity, radiative energy and radiative flux, for an arbitrary correlation function. A modified Gaussian probability distribution function is also used to average the solution in order to exclude the probable negative values of the optical variable. The problem is considered in half space medium which has specular reflecting boundary exposed to unit external incident flux. Numerical results of the average reflectivity, average radiant energy and average net flux are obtained for both Gaussian and modified Gaussian probability density functions at different degrees of polarization

Lactational transfer of mercury and polychlorinated biphenyls in polar bears.

Science.gov (United States)

Knott, Katrina K; Boyd, Daryle; Ylitalo, Gina M; O'Hara, Todd M

2012-07-01

We examined concentrations of total mercury (tHg, inorganic and methylated forms) and polychlorinated biphenyls (PCBs) in blood and milk from free-ranging Southern Beaufort-Chukchi Sea polar bears (Ursus maritimus) to assess maternal transfer of contaminants during lactation and the potential health risk to nursing young. Concentrations of contaminants in the blood of dependent and juvenile animals (ages 1-5 years) ranged from 35.9 to 52.2 μg kg(-1) ww for tHg and 13.9 to 52.2 μg kg(-1) ww (3255.81-11067.79 μg kg(-1) lw) for ΣPCB(7)s, similar to those of adult females, but greater than adult males. Contaminant concentrations in milk ranged from 5.7 to 71.8 μg tHg kg(-1)ww and 160 to 690 μg ΣPCB(11)s kg(-1) ww (547-5190 μg kg(-1) lw). The daily intake levels for tHg by milk consumption estimated for dependent young were below the tolerable daily intake level (TDIL) of tHg established for adult humans. Although the daily intake levels of PCBs through milk consumption for cubs of the year exceeded the TDIL thresholds, calculated dioxin equivalents for PCBs in milk were below adverse physiological thresholds for aquatic mammals. Relatively high concentrations of non-dioxin like PCBs in polar bear milk and blood could impact endocrine function of Southern Beaufort-Chukchi Sea polar bears, but this is uncertain. Transfer of contaminants during mid to late lactation likely limits bioaccumulation of dietary contaminants in female polar bears during spring. As polar bears respond to changes in their arctic sea ice habitat, the adverse health impacts associated with nutritional stress may be exacerbated by tHg and PCBs exposure, especially in ecologically and toxicologically sensitive polar bear cohorts such as reproductive females and young. Copyright © 2012. Published by Elsevier Ltd.

Analyzing powers and proton spin transfer coefficients in the elastic scattering of 800 MeV polarized protons from an L-type polarized deuteron target at small momentum transfers

International Nuclear Information System (INIS)

Adams, D.L.

1986-10-01

Analyzing powers and spin transfer coefficients which describe the elastic scattering of polarized protons from a polarized deuteron target have been measured. The energy of the proton beam was 800 MeV and data were taken at laboratory scattering angles of 7, 11, 14, and 16.5 degrees. One analyzing power was also measured at 180 degrees. Three linearly independent orientations of the beam polarization were used and the target was polarized parallel and antiparallel to the direction of the beam momentum. The data were taken with the high resolution spectrometer at the Los Alamos Meson Physics Facility (experiment 685). The results are compared with multiple scattering predictions based on Dirac representations of the nucleon-nucleon scattering matrices. 27 refs., 28 figs., 4 tabs

Polarization transfer in x-ray transitions due to photoionization in highly charged copper-like ions

Science.gov (United States)

Ma, Kun; Chen, Zhan-Bin; Xie, Lu-You; Dong, Chen-Zhong

2018-02-01

Using the density matrix theory and the multi-configuration Dirac-Fock method, the 3{d}3/2 subshell photoionization of highly charged ions is studied, together with their subsequent radiative decay. The effects of polarization transfer on the linear polarization and angular distribution of the 3{d}94{s}2{}2{D}3/2\\to 3{d}104p{}2{P}1/2 characteristic line photoemission for selected Cu-like Zn+, Ba27+, {{{W}}}45+, and {{{U}}}63+ ions are investigated. Our results show that the polarization transfer, arising from the originally polarized incident light, may lead to a considerable change in the alignment parameters and the polarization properties of the radiation, the character of which is highly sensitive to the initial photon polarization, yet virtually independent of the photon energy. These characteristics are very similar to those of the electron bremsstrahlung process reported by Märtin et al (2012 Phys. Rev. Lett. 108 264801). The present results are compared with available experimental results and show a good quantitative agreement.

Arcmancer: Geodesics and polarized radiative transfer library

Science.gov (United States)

Pihajoki, Pauli; Mannerkoski, Matias; Nättilä, Joonas; Johansson, Peter H.

2018-05-01

Arcmancer computes geodesics and performs polarized radiative transfer in user-specified spacetimes. The library supports Riemannian and semi-Riemannian spaces of any dimension and metric; it also supports multiple simultaneous coordinate charts, embedded geometric shapes, local coordinate systems, and automatic parallel propagation. Arcmancer can be used to solve various problems in numerical geometry, such as solving the curve equation of motion using adaptive integration with configurable tolerances and differential equations along precomputed curves. It also provides support for curves with an arbitrary acceleration term and generic tools for generating ray initial conditions and performing parallel computation over the image, among other tools.

Polarization tunable photogenerated carrier transfer of CH3NH3PbI3/polyvinylidene fluoride heterostructure

Science.gov (United States)

Yang, Kang; Deng, Zun-Yi; Feng, Hong-Jian

2017-10-01

The integration of ferroelectrics and organic-inorganic halide perovskites could be a promising way to facilitate the separation of electron-hole pairs and charge extraction for the application of solar cells. To explore the effect of the external ferroelectric layer on the CH3NH3PbI3 (MAPbI3) side, we perform first-principles calculations to study the charge transfer properties of the MAPbI3/polyvinylidene fluoride (PVDF) heterostructure. Our calculations demonstrate that the ferroelectric polarization pointing to the PVDF side can clearly facilitate the separation of photo-induced carriers and enhance charge extraction from MAPbI3, while opposite polarization direction hinders the charge extraction and collection. Notably, the carrier behavior at the interface is strongly tuned by the electric field associated with the ferroelectric polarization. In addition, excited state simulation confirms the tunable charge transfer of the MAPbI3/PVDF heterojunction. Therefore, the polarization-driven charge transfer mechanism provides a route for fabricating the ferroelectrics-based high-efficiency photovoltaics and switchable diode devices.

Spin transfers for baryon production in polarized pp collisions at RHIC-BNL

International Nuclear Information System (INIS)

Ma BoQiang; Schmidt, Ivan; Soffer, Jacques; Yang Jianjun

2002-01-01

We consider the inclusive production of longitudinally polarized baryons in p→p collisions at RHIC-BNL, with one longitudinally polarized proton. We study the spin transfer between the initial proton and the produced baryon as a function of its rapidity and we elucidate its sensitivity to the quark helicity distributions of the proton and to the polarized fragmentation functions of the quark into the baryon. We make predictions using an SU(6) quark spectator model and a perturbative QCD (pQCD) based model. We discuss these different predictions, and what can be learned from them, in view of the forthcoming experiments at RHIC-BNL

On the derivation of vector radiative transfer equation for polarized radiative transport in graded index media

International Nuclear Information System (INIS)

Zhao, J.M.; Tan, J.Y.; Liu, L.H.

2012-01-01

Light transport in graded index media follows a curved trajectory determined by Fermat's principle. Besides the effect of variation of the refractive index on the transport of radiative intensity, the curved ray trajectory will induce geometrical effects on the transport of polarization ellipse. This paper presents a complete derivation of vector radiative transfer equation for polarized radiation transport in absorption, emission and scattering graded index media. The derivation is based on the analysis of the conserved quantities for polarized light transport along curved trajectory and a novel approach. The obtained transfer equation can be considered as a generalization of the classic vector radiative transfer equation that is only valid for uniform refractive index media. Several variant forms of the transport equation are also presented, which include the form for Stokes parameters defined with a fixed reference and the Eulerian forms in the ray coordinate and in several common orthogonal coordinate systems.

Polar transfer alignment of shipborne SINS with a large misalignment angle

International Nuclear Information System (INIS)

Cheng, Jianhua; Wang, Tongda; Guan, Dongxue; Li, Meiling

2016-01-01

Existing polar transfer alignment (TA) algorithms are designed based on linear Kalman filters (KF) to estimate misalignment angles. In the case of a large misalignment angle, these algorithms cannot be applied in order to achieve accurate TA. In this paper, a TA algorithm based on an unscented Kalman filter (UKF) is proposed to solve the problem of the large misalignment angle in the polar region. Based on a large misalignment angle, nonlinear navigation error equations, which are the UKF dynamic models, are derived under grid frames. This paper chooses the velocity plus attitude matching method as the TA matching method and errors of velocity and attitude as observations. The misalignment angle can be estimated by the designed UKF. The simulation results have demonstrated that the polar TA algorithm can be effective in improving the TA accuracy, especially when large misalignment angles occur. (paper)

Multiple scattering of polarized light: comparison of Maxwell theory and radiative transfer theory.

Science.gov (United States)

Voit, Florian; Hohmann, Ansgar; Schäfer, Jan; Kienle, Alwin

2012-04-01

For many research areas in biomedical optics, information about scattering of polarized light in turbid media is of increasing importance. Scattering simulations within this field are mainly performed on the basis of radiative transfer theory. In this study a polarization sensitive Monte Carlo solution of radiative transfer theory is compared to exact Maxwell solutions for all elements of the scattering Müller matrix. Different scatterer volume concentrations are modeled as a multitude of monodisperse nonabsorbing spheres randomly positioned in a cubic simulation volume which is irradiated with monochromatic incident light. For all Müller matrix elements effects due to dependent scattering and multiple scattering are analysed. The results are in overall good agreement between the two methods with deviations related to dependent scattering being prominent for high volume concentrations and high scattering angles.

Live births after polar body biopsy and frozen-thawed cleavage stage embryo transfer: case report.

Science.gov (United States)

Guimarães, Fernando; Roque, Matheus; Valle, Marcello; Kostolias, Alessandra; Azevedo, Rodrigo A de; Martinhago, Ciro D; Sampaio, Marcos; Geber, Selmo

2016-12-01

Pre-implantation genetic diagnosis (PGD) or screening (PGS) technology, has emerged and developed in the past few years, benefiting couples as it allows the selection and transfer of healthy embryos during IVF treatments. These techniques can be performed in oocytes (polar-body biopsy) or embryos (blastomere or trophectoderm biopsy). In this case report, we describe the first two live births to be published in Brazil after a polar-body (PB) biopsy. In case 1, a 42-year-old was submitted to PB biopsy with PGS due to advanced maternal age and poor ovarian reserve. Five MII oocytes underwent first and second polar body biopsy and four cleavage embryos were cryopreserved. The PGS analysis resulted in two euploid embryos (next generation sequence). A frozen-thawed embryo transfer (FET) was performed after endometrial priming and a healthy baby was delivered after a cesarean section (37 weeks, female, 3390g, 47.5 cm). In case 2, a 40-year old patient with balanced translocation and poor ovarian response was submitted to PB biopsy. Two MII oocytes underwent first and second polar body biopsy and two embryos were cryopreserved in cleavage stage. The analysis resulted in one euploid embryo that was transferred after endometrial priming. A preterm healthy baby (34 weeks, female, 2100g, 40 cm) was delivered via cesarean section. In conclusion, although the blastocyst biopsy is the norm when performing PGS/PGD during IVF treatments, other alternatives (as PB biopsy) should be considered in some specific situations.

Formal Solutions for Polarized Radiative Transfer. II. High-order Methods

Energy Technology Data Exchange (ETDEWEB)

Janett, Gioele; Steiner, Oskar; Belluzzi, Luca, E-mail: gioele.janett@irsol.ch [Istituto Ricerche Solari Locarno (IRSOL), 6605 Locarno-Monti (Switzerland)

2017-08-20

When integrating the radiative transfer equation for polarized light, the necessity of high-order numerical methods is well known. In fact, well-performing high-order formal solvers enable higher accuracy and the use of coarser spatial grids. Aiming to provide a clear comparison between formal solvers, this work presents different high-order numerical schemes and applies the systematic analysis proposed by Janett et al., emphasizing their advantages and drawbacks in terms of order of accuracy, stability, and computational cost.

Alfven waves in dusty plasmas with plasma particles described by anisotropic kappa distributions

Energy Technology Data Exchange (ETDEWEB)

Galvao, R. A.; Ziebell, L. F. [Instituto de Fisica, Universidade Federal do Rio Grande do Sul, Caixa Postal 15051, CEP: 91501-970, Porto Alegre, Rio Grande do Sul (Brazil); Gaelzer, R. [Instituto de Fisica e Matematica, Universidade Federal de Pelotas, Caixa Postal 354-Campus UFPel, CEP: 96010-900 Pelotas, Rio Grande do Sul (Brazil); Juli, M. C. de [Centro de Radio-Astronomia e Astrofisica Mackenzie-CRAAM, Universidade Presbiteriana Mackenzie, Rua da Consolacao 896, CEP: 01302-907 Sao Paulo, Sao Paulo (Brazil)

2012-12-15

We utilize a kinetic description to study the dispersion relation of Alfven waves propagating parallelly to the ambient magnetic field in a dusty plasma, taking into account the fluctuation of the charge of the dust particles, which is due to inelastic collisions with electrons and ions. We consider a plasma in which the velocity distribution functions of the plasma particles are modelled as anisotropic kappa distributions, study the dispersion relation for several combinations of the parameters {kappa}{sub Parallel-To} and {kappa}{sub Up-Tack }, and emphasize the effect of the anisotropy of the distributions on the mode coupling which occurs in a dusty plasma, between waves in the branch of circularly polarized waves and waves in the whistler branch.

Joule heating and spin-transfer torque investigated on the atomic scale using a spin-polarized scanning tunneling microscope.

Science.gov (United States)

Krause, S; Herzog, G; Schlenhoff, A; Sonntag, A; Wiesendanger, R

2011-10-28

The influence of a high spin-polarized tunnel current onto the switching behavior of a superparamagnetic nanoisland on a nonmagnetic substrate is investigated by means of spin-polarized scanning tunneling microscopy. A detailed lifetime analysis allows for a quantification of the effective temperature rise of the nanoisland and the modification of the activation energy barrier for magnetization reversal, thereby using the nanoisland as a local thermometer and spin-transfer torque analyzer. Both the Joule heating and spin-transfer torque are found to scale linearly with the tunnel current. The results are compared to experiments performed on lithographically fabricated magneto-tunnel junctions, revealing a very high spin-transfer torque switching efficiency in our experiments.

Polarization transfer between oriented metastable helium atoms and neon atoms. A comparison of even and odd isotopes

Energy Technology Data Exchange (ETDEWEB)

Pepper, D M; Wang, H T.M.

1983-11-01

Collision-induced polarization transfer from optically pumped helium to excited states of neon is studied using various combinations of even and odd isotopes. It is found that, within our experimental accuracy of 10%, the resultant polarization is independent of the isotopic composition of the binary mixture. Possible applications using this mechanism are discussed.

Formal Solutions for Polarized Radiative Transfer. I. The DELO Family

Energy Technology Data Exchange (ETDEWEB)

Janett, Gioele; Carlin, Edgar S.; Steiner, Oskar; Belluzzi, Luca, E-mail: gioele.janett@irsol.ch [Istituto Ricerche Solari Locarno (IRSOL), 6605 Locarno-Monti (Switzerland)

2017-05-10

The discussion regarding the numerical integration of the polarized radiative transfer equation is still open and the comparison between the different numerical schemes proposed by different authors in the past is not fully clear. Aiming at facilitating the comprehension of the advantages and drawbacks of the different formal solvers, this work presents a reference paradigm for their characterization based on the concepts of order of accuracy , stability , and computational cost . Special attention is paid to understand the numerical methods belonging to the Diagonal Element Lambda Operator family, in an attempt to highlight their specificities.

Improper ferroelectric polarization in a perovskite driven by intersite charge transfer and ordering

Science.gov (United States)

Chen, Wei-Tin; Wang, Chin-Wei; Wu, Hung-Cheng; Chou, Fang-Cheng; Yang, Hung-Duen; Simonov, Arkadiy; Senn, M. S.

2018-04-01

It is of great interest to design and make materials in which ferroelectric polarization is coupled to other order parameters such as lattice, magnetic, and electronic instabilities. Such materials will be invaluable in next-generation data storage devices. Recently, remarkable progress has been made in understanding improper ferroelectric coupling mechanisms that arise from lattice and magnetic instabilities. However, although theoretically predicted, a compact lattice coupling between electronic and ferroelectric (polar) instabilities has yet to be realized. Here we report detailed crystallographic studies of a perovskite HgAMn3A'Mn4BO12 that is found to exhibit a polar ground state on account of such couplings that arise from charge and orbital ordering on both the A'- and B-sites, which are themselves driven by a highly unusual MnA '-MnB intersite charge transfer. The inherent coupling of polar, charge, orbital, and hence magnetic degrees of freedom make this a system of great fundamental interest, and demonstrating ferroelectric switching in this and a host of recently reported hybrid improper ferroelectrics remains a substantial challenge.

The evolution of tensor polarization

International Nuclear Information System (INIS)

Huang, H.; Lee, S.Y.; Ratner, L.

1993-01-01

By using the equation of motion for the vector polarization, the spin transfer matrix for spin tensor polarization, the spin transfer matrix for spin tensor polarization is derived. The evolution equation for the tensor polarization is studied in the presence of an isolate spin resonance and in the presence of a spin rotor, or snake

Spin Transfer in Inclusive Λ0 Production by Transversely Polarized Protons at 200GeV/c

International Nuclear Information System (INIS)

Grosnick, D.P.; Hill, D.A.; Laghai, M.; Lopiano, D.; Ohashi, Y.; Spinka, H.; Stanek, R.W.; Underwood, D.G.; Yokosawa, A.; Bystricky, J.; Lehar, F.; Lesquen, A. de; Rossum, L. van; Cossairt, J.D.; Read, A.L.; Iwatani, K.; Belikov, N.I.; Derevschikov, A.A.; Grachov, O.A.; Matulenko, Y.A.; Meschanin, A.P.; Nurushev, S.B.; Patalakha, D.I.; Rykov, V.L.; Solovyanov, V.L.; Vasiliev, A.N.; Akchurin, N.; Onel, Y.; Maki, T.; Enyo, H.; Funahashi, H.; Goto, Y.; Iijima, T.; Imai, K.; Itow, Y.; Makino, S.; Masaike, A.; Miyake, K.; Nagamine, T.; Saito, N.; Yamashita, S.; Takashima, R.; Takeutchi, F.; Kuroda, K.; Michalowicz, A.; Rappazzo, G.F.; Salvato, G.; Luehring, F.C.; Miller, D.H.; Tamura, N.; Yoshida, T.; Adams, D.L.; Bonner, B.E.; Corcoran, M.D.; Cranshaw, J.; Nessi-Tedaldi, F.; Nessi, M.; Nguyen, C.; Roberts, J.B.; Skeens, J.; White, J.L.; Bravar, A.

1997-01-01

Surprisingly large polarizations in hyperon production by unpolarized protons have been known for a long time. The spin dynamics of the production process can be further investigated with polarized beams. Recently, a negative asymmetry A N was found in inclusive Λ 0 production with a 200GeV/c transversely polarized proton beam. The depolarization D NN in p↑+p→Λ 0 +X has been measured with the same beam over a wide x F range and at moderate p T . D NN reaches positive values of about 30% at high x F and p T ∼1.0GeV/c . This result shows a sizable spin transfer from the incident polarized proton to the outgoing Λ 0 . copyright 1997 The American Physical Society

Considering polarization in MODIS-based cloud property retrievals by using a vector radiative transfer code

International Nuclear Information System (INIS)

Yi, Bingqi; Huang, Xin; Yang, Ping; Baum, Bryan A.; Kattawar, George W.

2014-01-01

In this study, a full-vector, adding–doubling radiative transfer model is used to investigate the influence of the polarization state on cloud property retrievals from Moderate Resolution Imaging Spectroradiometer (MODIS) satellite observations. Two sets of lookup tables (LUTs) are developed for the retrieval purposes, both of which provide water cloud and ice cloud reflectivity functions at two wavelengths in various sun-satellite viewing geometries. However, only one of the LUTs considers polarization. The MODIS reflectivity observations at 0.65 μm (band 1) and 2.13 μm (band 7) are used to infer the cloud optical thickness and particle effective diameter, respectively. Results indicate that the retrievals for both water cloud and ice cloud show considerable sensitivity to polarization. The retrieved water and ice cloud effective diameter and optical thickness differences can vary by as much as ±15% due to polarization state considerations. In particular, the polarization state has more influence on completely smooth ice particles than on severely roughened ice particles. - Highlights: • Impact of polarization on satellite-based retrieval of water/ice cloud properties is studied. • Inclusion of polarization can change water/ice optical thickness and effective diameter values by up to ±15%. • Influence of polarization on cloud property retrievals depends on sun-satellite viewing geometries

The Physics of Polarization

Science.gov (United States)

Landi Degl'Innocenti, Egidio

2015-10-01

The introductory lecture that has been delivered at this Symposium is a condensed version of an extended course held by the author at the XII Canary Island Winter School from November 13 to November 21, 2000. The full series of lectures can be found in Landi Degl'Innocenti (2002). The original reference is organized in 20 Sections that are here itemized: 1. Introduction, 2. Description of polarized radiation, 3. Polarization and optical devices: Jones calculus and Muller matrices, 4. The Fresnel equations, 5. Dichroism and anomalous dispersion, 6. Polarization in everyday life, 7. Polarization due to radiating charges, 8. The linear antenna, 9. Thomson scattering, 10. Rayleigh scattering, 11. A digression on Mie scattering, 12. Bremsstrahlung radiation, 13. Cyclotron radiation, 14. Synchrotron radiation, 15. Polarization in spectral lines, 16. Density matrix and atomic polarization, 17. Radiative transfer and statistical equilibrium equations, 18. The amplification condition in polarized radiative transfer, and 19. Coupling radiative transfer and statistical equilibrium equations.

RADIATIVE TRANSFER MODELING OF THE ENIGMATIC SCATTERING POLARIZATION IN THE SOLAR Na i D{sub 1} LINE

Energy Technology Data Exchange (ETDEWEB)

Belluzzi, Luca [Istituto Ricerche Solari Locarno, CH-6605 Locarno Monti (Switzerland); Bueno, Javier Trujillo [Instituto de Astrofísica de Canarias, E-38205 La Laguna, Tenerife (Spain); Degl’Innocenti, Egidio Landi [Dipartimento di Fisica e Astronomia, Università di Firenze, I-50125 Firenze (Italy)

2015-12-01

The modeling of the peculiar scattering polarization signals observed in some diagnostically important solar resonance lines requires the consideration of the detailed spectral structure of the incident radiation field as well as the possibility of ground level polarization, along with the atom's hyperfine structure and quantum interference between hyperfine F-levels pertaining either to the same fine structure J-level, or to different J-levels of the same term. Here we present a theoretical and numerical approach suitable for solving this complex non-LTE radiative transfer problem. This approach is based on the density-matrix metalevel theory (where each level is viewed as a continuous distribution of sublevels) and on accurate formal solvers of the transfer equations and efficient iterative methods. We show an application to the D-lines of Na i, with emphasis on the enigmatic D{sub 1} line, pointing out the observable signatures of the various physical mechanisms considered. We demonstrate that the linear polarization observed in the core of the D{sub 1} line may be explained by the effect that one gets when the detailed spectral structure of the anisotropic radiation responsible for the optical pumping is taken into account. This physical ingredient is capable of introducing significant scattering polarization in the core of the Na i D{sub 1} line without the need for ground-level polarization.

BACKWARD AND FORWARD MONTE CARLO METHOD IN POLARIZED RADIATIVE TRANSFER

Energy Technology Data Exchange (ETDEWEB)

Yong, Huang; Guo-Dong, Shi; Ke-Yong, Zhu, E-mail: huangy_zl@263.net [School of Aeronautical Science and Engineering, Beihang University, Beijing 100191 (China)

2016-03-20

In general, the Stocks vector cannot be calculated in reverse in the vector radiative transfer. This paper presents a novel backward and forward Monte Carlo simulation strategy to study the vector radiative transfer in the participated medium. A backward Monte Carlo process is used to calculate the ray trajectory and the endpoint of the ray. The Stocks vector is carried out by a forward Monte Carlo process. A one-dimensional graded index semi-transparent medium was presented as the physical model and the thermal emission consideration of polarization was studied in the medium. The solution process to non-scattering, isotropic scattering, and the anisotropic scattering medium, respectively, is discussed. The influence of the optical thickness and albedo on the Stocks vector are studied. The results show that the U, V-components of the apparent Stocks vector are very small, but the Q-component of the apparent Stocks vector is relatively larger, which cannot be ignored.

Imaging and modeling of collagen architecture in living tissue with polarized light transfer (Conference Presentation)

Science.gov (United States)

Ramella-Roman, Jessica C.; Stoff, Susan; Chue-Sang, Joseph; Bai, Yuqiang

2016-03-01

The extra-cellular space in connective tissue of animals and humans alike is comprised in large part of collagen. Monitoring of collagen arrangement and cross-linking has been utilized to diagnose a variety of medical conditions and guide surgical intervention. For example, collagen monitoring is useful in the assessment and treatment of cervical cancer, skin cancer, myocardial infarction, and non-arteritic anterior ischemic optic neuropathy. We have developed a suite of tools and models based on polarized light transfer for the assessment of collagen presence, cross-linking, and orientation in living tissue. Here we will present some example of such approach applied to the human cervix. We will illustrate a novel Mueller Matrix (MM) imaging system for the study of cervical tissue; furthermore we will show how our model of polarized light transfer through cervical tissue compares to the experimental findings. Finally we will show validation of the methodology through histological results and Second Harmonic imaging microscopy.

Polarization transfer in the 3H(rvec p,rvec n)3He reaction and the 0- level in 4He

International Nuclear Information System (INIS)

Walston, J.R.; Gould, C.R.; Haase, D.G.; Raichle, B.W.; Seely, M.L.; Walston, J.R.; Keith, C.D.; Gould, C.R.; Haase, D.G.; Raichle, B.W.; Seely, M.L.; Tornow, W.; Wilburn, W.S.; Keith, C.D.; Tornow, W.; Wilburn, W.S.; Hoffmann, G.W.; Penttilae, S.I.

1998-01-01

Longitudinal polarization-transfer coefficients for the 3 H(rvec p,rvec n) 3 He reaction have been measured at zero degrees for proton energies of 1.3 endash 2.8 MeV. The results show a striking resonance behavior for energies corresponding to excitation of the 0 - level in 4 He at 21.0 MeV. In agreement with R-matrix calculations, the value approaches unity at 1.52 MeV, the peak of the resonance. Near this same energy, at 1.62 MeV, the transverse polarization-transfer coefficient was measured to be consistent with zero. copyright 1998 The American Physical Society

A MULTIPLE SCATTERING POLARIZED RADIATIVE TRANSFER MODEL: APPLICATION TO HD 189733b

Energy Technology Data Exchange (ETDEWEB)

Kopparla, Pushkar; Yung, Yuk L. [Division of Geological and Planetary Sciences, California Institute of Technology, Pasadena, CA (United States); Natraj, Vijay; Swain, Mark R. [Jet Propulsion Laboratory (NASA-JPL), Pasadena, CA (United States); Zhang, Xi [Lunar and Planetary Laboratory, University of Arizona, Tucson, AZ (United States); Wiktorowicz, Sloane J., E-mail: pkk@gps.caltech.edu [Department of Astronomy and Astrophysics, University of California, Santa Cruz, CA (United States)

2016-01-20

We present a multiple scattering vector radiative transfer model that produces disk integrated, full phase polarized light curves for reflected light from an exoplanetary atmosphere. We validate our model against results from published analytical and computational models and discuss a small number of cases relevant to the existing and possible near-future observations of the exoplanet HD 189733b. HD 189733b is arguably the most well observed exoplanet to date and the only exoplanet to be observed in polarized light, yet it is debated if the planet’s atmosphere is cloudy or clear. We model reflected light from clear atmospheres with Rayleigh scattering, and cloudy or hazy atmospheres with Mie and fractal aggregate particles. We show that clear and cloudy atmospheres have large differences in polarized light as compared to simple flux measurements, though existing observations are insufficient to make this distinction. Futhermore, we show that atmospheres that are spatially inhomogeneous, such as being partially covered by clouds or hazes, exhibit larger contrasts in polarized light when compared to clear atmospheres. This effect can potentially be used to identify patchy clouds in exoplanets. Given a set of full phase polarimetric measurements, this model can constrain the geometric albedo, properties of scattering particles in the atmosphere, and the longitude of the ascending node of the orbit. The model is used to interpret new polarimetric observations of HD 189733b in a companion paper.

Neutron polarization in polarized 3He targets

International Nuclear Information System (INIS)

Friar, J.L.; Gibson, B.F.; Payne, G.L.; Bernstein, A.M.; Chupp, T.E.

1990-01-01

Simple formulas for the neutron and proton polarizations in polarized 3 He targets are derived assuming (1) quasielastic final states; (2) no final-state interactions; (3) no meson-exchange currents; (4) large momentum transfers; (5) factorizability of 3 He SU(4) response-function components. Numerical results from a wide variety of bound-state solutions of the Faddeev equations are presented. It is found that this simple model predicts the polarization of neutrons in a fully polarized 3 He target to be 87%, while protons should have a slight residual polarization of -2.7%. Numerical studies show that this model works very well for quasielastic electron scattering

Polarized scattered light from self-luminous exoplanets. Three-dimensional scattering radiative transfer with ARTES

Science.gov (United States)

Stolker, T.; Min, M.; Stam, D. M.; Mollière, P.; Dominik, C.; Waters, L. B. F. M.

2017-11-01

Context. Direct imaging has paved the way for atmospheric characterization of young and self-luminous gas giants. Scattering in a horizontally-inhomogeneous atmosphere causes the disk-integrated polarization of the thermal radiation to be linearly polarized, possibly detectable with the newest generation of high-contrast imaging instruments. Aims: We aim to investigate the effect of latitudinal and longitudinal cloud variations, circumplanetary disks, atmospheric oblateness, and cloud particle properties on the integrated degree and direction of polarization in the near-infrared. We want to understand how 3D atmospheric asymmetries affect the polarization signal in order to assess the potential of infrared polarimetry for direct imaging observations of planetary-mass companions. Methods: We have developed a three-dimensional Monte Carlo radiative transfer code (ARTES) for scattered light simulations in (exo)planetary atmospheres. The code is applicable to calculations of reflected light and thermal radiation in a spherical grid with a parameterized distribution of gas, clouds, hazes, and circumplanetary material. A gray atmosphere approximation is used for the thermal structure. Results: The disk-integrated degree of polarization of a horizontally-inhomogeneous atmosphere is maximal when the planet is flattened, the optical thickness of the equatorial clouds is large compared to the polar clouds, and the clouds are located at high altitude. For a flattened planet, the integrated polarization can both increase or decrease with respect to a spherical planet which depends on the horizontal distribution and optical thickness of the clouds. The direction of polarization can be either parallel or perpendicular to the projected direction of the rotation axis when clouds are zonally distributed. Rayleigh scattering by submicron-sized cloud particles will maximize the polarimetric signal whereas the integrated degree of polarization is significantly reduced with micron

Wideband metamaterial array with polarization-independent and wide incident angle for harvesting ambient electromagnetic energy and wireless power transfer

Science.gov (United States)

Zhong, Hui-Teng; Yang, Xue-Xia; Song, Xing-Tang; Guo, Zhen-Yue; Yu, Fan

2017-11-01

In this work, we introduced the design, demonstration, and discussion of a wideband metamaterial array with polarization-independent and wide-angle for harvesting ambient electromagnetic (EM) energy and wireless power transfer. The array consists of unit cells with one square ring and four metal bars. In comparison to the published metamaterial arrays for harvesting EM energy or wireless transfer, this design had the wide operation bandwidth with the HPBW (Half Power Band Width) of 110% (6.2 GHz-21.4 GHz), which overcomes the narrow-band operation induced by the resonance characteristic of the metamaterial. On the normal incidence, the simulated maximum harvesting efficiency was 96% and the HPBW was 110% for the random polarization wave. As the incident angle increases to 45°, the maximum efficiency remained higher than 88% and the HPBW remained higher than 83% for the random polarization wave. Furthermore, the experimental verification of the designed metamaterial array was conducted, and the measured results were in reasonable agreement with the simulated ones.

H- ion current from a polarized vapor target

International Nuclear Information System (INIS)

Cornelius, W.D.

1984-01-01

A method of determining the polarization transferred to hydrogen atoms in charge-exchange reactions is outlined. The method also provides a means of determining target polarizations once the polarization transfer function is known

Transient-field strength measurements for 52Cr traversing Fe hosts at high velocity and polarization transfer mechanisms

International Nuclear Information System (INIS)

Stuchbery, A.E.; Doran, C.E.; Byrne, A.P.; Bolotin, H.H.; Dracoulis, G.D.

1986-12-01

Transient-field strengths were measured for 52 Cr ions traversing polarized Fe hosts at velocities up to 12v>=o (v>=o = c/137 = Bohr velocity). The results are compared with predictions of various transient field parametrizations and discussed in terms of possible mechanisms by which polarization might be transferred from the Fe host to inner vacancies of the moving Cr ions. The g-factor of the first 2 + state of 52 Cr was also measured by the transient field technique and found to be in accord with shell-model calculations

Photoinduced electron transfer in covalent ruthenium-anthraquinone dyads: relative importance of driving-force, solvent polarity, and donor-bridge energy gap.

Science.gov (United States)

Hankache, Jihane; Wenger, Oliver S

2012-02-28

Four rigid rod-like molecules comprised of a Ru(bpy)(3)(2+) (bpy = 2,2'-bipyridine) photosensitizer, a 9,10-anthraquinone electron acceptor, and a molecular bridge connecting the two redox partners were synthesized and investigated by optical spectroscopic and electrochemical means. An attempt was made to assess the relative importance of driving-force, solvent polarity, and bridge variation on the rates of photoinduced electron transfer in these molecules. Expectedly, introduction of tert-butyl substituents in the bipyridine ligands of the ruthenium complex and a change in solvent from dichloromethane to acetonitrile lead to a significant acceleration of charge transfer rates. In dichloromethane, photoinduced electron transfer is not competitive with the inherent excited-state deactivation processes of the photosensitizer. In acetonitrile, an increase in driving-force by 0.2 eV through attachment of tert-butyl substituents to the bpy ancillary ligands causes an increase in electron transfer rates by an order of magnitude. Replacement of a p-xylene bridge by a p-dimethoxybenzene spacer entails an acceleration of charge transfer rates by a factor of 3.5. In the dyads from this study, the relative order of importance of individual influences on electron transfer rates is therefore as follows: solvent polarity ≥ driving-force > donor-bridge energy gap.

Nuclear polarization potential due to particle transfer in heavy-ion collisions

International Nuclear Information System (INIS)

Landowne, S.; Dasso, C.H.; Winther, A.; Pollarolo, G.

1986-01-01

The effective interaction which determines the elastic scattering of heavy composite systems consists of a ''bare'' real potential V, noramally identified with the folding model, a renormalization term or ''polarization potential'' ΔV and an imaginary ''absorptive potential'' iW. The latter contributions originate from the couplings to intrinsic degrees of freedom. While iW is a conspicuous feature of all optical model analyses, the related term ΔV has received relatively little attention until recently. The microscopic structure of ΔV + iW is examined using second-order semi-classical perturbation theory. Focus is on the long-range part of ΔV which is governed by single-particle transfer reactions between the colliding systems

Nuclear polarization potential due to particle transfer in heavy-ion collisions

International Nuclear Information System (INIS)

Landowne, S.; Dasso, C.H.; Winther, A.; Pollarolo, G.

1986-01-01

The effective interaction which determines the elastic scattering of heavy composite systems consists of a bare real potential V, normally identified with the folding model, a renormalization term or polarization potential ΔV and an imaginary absorptive potential iW. The latter contributions originate from the couplings to intrinsic degrees of freedom. While iW is a conspicuous feature of all optical model analyses, the related term ΔV has received relatively little attention until recently. Here the authors examine the microscopic structure of ΔV + IW using second-order semi-classical perturbation theory. In particular, they focus on the long-range part of ΔV which is governed by single-particle transfer reactions between the colliding systems

Study of nuclear isovector spin responses from polarization transfer in (p,n) reactions at intermediate energies

International Nuclear Information System (INIS)

Wakasa, Tomotsugu

1997-01-01

We have measured a complete set of polarization transfer observables has been measured for quasi-free (p vector, n vector) reactions on 2 H, 6 Li, 12 C, 40 Ca, and 208 Pb at a bombarding energy of 346MeV and a laboratory scattering angle of 22deg (q=1.7 fm -1 ). The polarization transfer observables for all five targets are remarkably similar. These polarization observables yield separated spin-longitudinal (σ·q) and spin-transverse (σxq) nuclear responses. These results are compared to the spin-transverse responses measured in deep-inelastic electron scattering as well as to nuclear responses based on the random phase approximation. Such a comparison reveals an enhancement in the (p vector, n vector) spin-transverse channel, which masks the effect of pionic correlations in the response ratio. Second, the double differential cross sections at θ lab between 0deg and 12.3deg and the polarization transfer D NN at 0deg for the 90 Zr(p,n) reaction are measured at a bombarding energy of 295MeV. The Gamow-Teller(GT) strength B(GT) in the continuum deduced from the L=0 cross section is compared both with the perturbative calculation by Bertsch and Hamamoto and with the second-order random phase approximation calculation by Drozdz et al. The sum of B(GT) values up to 50MeV excitation becomes S β- =28.0±1.6 after subtracting the contribution of the isovector spin-monopole strength. This S β- value of 28.0±1.6 corresponds to about (93±5)% of the minimum value of the sum-rule 3(N-Z)=30. Last, first measurements of D NN (0deg) for (p vector, n vector) reactions at 295MeV yield large negative values up to 50MeV excitation for the 6 Li, 11 B, 12 C, 13 C(p vector, n vector) reactions. DWIA calculations using the Franey and Love (FL) 270MeV interaction reproduce differential cross sections and D NN (0deg) values, while the FL 325MeV interaction yield D NN (0deg) values less negative than the experimental values. (J.P.N.)

Matrix formulations of radiative transfer including the polarization effect in a coupled atmosphere-ocean system

International Nuclear Information System (INIS)

Ota, Yoshifumi; Higurashi, Akiko; Nakajima, Teruyuki; Yokota, Tatsuya

2010-01-01

A vector radiative transfer model has been developed for a coupled atmosphere-ocean system. The radiative transfer scheme is based on the discrete ordinate and matrix operator methods. The reflection/transmission matrices and source vectors are obtained for each atmospheric or oceanic layer through the discrete ordinate solution. The vertically inhomogeneous system is constructed using the matrix operator method, which combines the radiative interaction between the layers. This radiative transfer scheme is flexible for a vertically inhomogeneous system including the oceanic layers as well as the ocean surface. Compared with the benchmark results, the computational error attributable to the radiative transfer scheme has been less than 0.1% in the case of eight discrete ordinate directions. Furthermore, increasing the number of discrete ordinate directions has produced computations with higher accuracy. Based on our radiative transfer scheme, simulations of sun glint radiation have been presented for wavelengths of 670 nm and 1.6 μm. Results of simulations have shown reasonable characteristics of the sun glint radiation such as the strongly peaked, but slightly smoothed radiation by the rough ocean surface and depolarization through multiple scattering by the aerosol-loaded atmosphere. The radiative transfer scheme of this paper has been implemented to the numerical model named Pstar as one of the OpenCLASTR/STAR radiative transfer code systems, which are widely applied to many radiative transfer problems, including the polarization effect.

Measurement of Tensor Polarization in Elastic Electron-Deuteron Scattering at Large Momentum Transfer

International Nuclear Information System (INIS)

David Abbott; Abdellah Ahmidouch; Heinz Anklin; Francois Arvieux; Jacques Ball; Beedoe, S.; Elizabeth Beise; Louis Bimbot; Werner Boeglin; Herbert Breuer; Roger Carlini; Nicholas Chant; Samuel Danagoulian; Dow, K.; Jean-Eric Ducret; James Dunne; Lars Ewell; Laurent Eyraud; Christophe Furget; Michel Garcon; Ronald Gilman; Charles Glashausser; Paul Gueye; Kenneth Gustafsson; Kawtar Hafidi; Adrian Honegger; Juerg Jourdan; Serge Kox; Gerfried Kumbartzki; Lu, L.; Allison Lung; David Mack; Pete Markowitz; Justin McIntyre; David Meekins; Fernand Merchez; Joseph Mitchell; Mohring, R.; Sekazi Mtingwa; Hamlet Mkrtchyan; David Pitz; Liming Qin; Ronald Ransome; Jean-Sebastien Real; Philip Roos; Paul Rutt; Reyad Sawafta; Samuel Stepanyan; Raphael Tieulent; Egle Tomasi-Gustafsson; William Turchinetz; Kelley Vansyoc; Jochen Volmer; Eric Voutier; William Vulcan; Claude Williamson; Stephen Wood; Chen Yan; Jie Zhao; Wenxia Zhao

2000-01-01

Tensor polarization observables (t20, t21 and t22) have been measured in elastic electron-deuteron scattering for six values of momentum transfer between 0.66 and 1.7 (GeV/c) 2 . The experiment was performed at the Jefferson Laboratory in Hall C using the electron HMS Spectrometer, a specially designed deuteron magnetic channel and the recoil deuteron polarimeter POLDER. The new data determine to much larger Q 2 the deuteron charge form factors G C and G Q . They are in good agreement with relativistic calculations and disagree with pQCD predictions

Polarization transfer in elastic p-d scattering at E sub. rho. = 22. 7 MeV

Energy Technology Data Exchange (ETDEWEB)

Gruebler, W.; Clajus, M.; Egun, P.M.; Hautle, P.; Weber, A. (Eidgenoessische Technische Hochschule, Zurich (CH). Inst. fuer Mittelenergiephysik); Schmelzbach, P.A. (Paul Scherrer Inst. (PSI), Villigen (CH)); Slaus, I. (Institut Ruder Boskovic, Zagreb. (YU)); Vuaridel, B. (Michigan Univ., Ann Arbor, MI (US)); Sperisen, F. (Indiana Univ. Cyclotron Facility, Bloomington, IN (US)); Kretschmer, W.; Karschnick, R.O.; Rauscher, A.; Weidmann, R.; Walter, T. (Erlangen-Nuernberg Univ., Erlangen (DE). Physikalisches Inst.); Bruno, M.; Cannata, F.; d' Agostino, M. (Istituto Nazionale di Fisica Nucleare, Bologna (IT))

1990-11-15

The proton-deuteron elastic scattering has been investigated at E{sub p}=22.7 MeV by comparison of rigorous Faddeev calculations with experimental results. From the calculations it was found that polarization transfer coefficients are more sensitive to details of the nucleon-nucleon potentials than the analyzing powers. Therefore we measured the proton to proton transfer coefficients K{sup y'}{sub y} and K{sup x'}{sub z}. The observable most sensitive to the tensor force is K{sup y'}{sub y}. The angular distributions of K{sup y'}{sub y} and, to a smaller extent, K{sup x'}{sub z} clearly favour the Bonn A potential.

Polarization Measurements in High-Energy Deuteron Photodisintegration

International Nuclear Information System (INIS)

Adam Sarty; Andrei Afanasev; Arunava Saha; Bogdan Wojtsekhowski; Brendan Fox; Chang, C.; Cathleen Jones; Charles Glashausser; Charles Perdrisat; Cornelis De Jager; Cornelis De Jager; Cornelis de Jager; Crovelli, D.; Daniel Simon; David Meekins; Demetrius Margaziotis; Dipangkar Dutta; Edgar Kooijman; Edward Brash; Edward Kinney; Elaine Schulte; Eugene Chudakov; Feng Xiong; Franco Garibaldi; Garth Huber; Gerfried Kumbartzki; Guido Urciuoli; Haiyan Gao; James Kelly; Javier Gomez; Jens-Ole Hansen; Jian-Ping Chen; John Calarco; John LeRose; Jordan Hovdebo; Joseph Mitchell; Juncai Gao; Kamal Benslama; Kathy McCormick; Kevin Fissum; Konrad Aniol; Krishni Wijesooriya; Louis Bimbot; Ludyvine Morand; Luminita Todor; Marat Rvachev; Mark Jones; Martin Epstein; Meihua Liang; Michael Kuss; Moskov Amarian; Nilanga Liyanage; Oleksandr Glamazdin; Olivier Gayou; Paul Ulmer; Pete Markowitz; Peter Bosted; Holt, R.; Riad Suleiman; Richard Lindgren; Rikki Roche; Robert Michaels; Roman Pomatsalyuk; Ronald Gilman; Ronald Ransome; Salvatore Frullani; Scott Dumalski; Seonho Choi; Sergey Malov; Sonja Dieterich; Steffen Strauch; Stephen Becher; Steve Churchwell; Ting Chang; Viktor Gorbenko; Vina Punjabi; Xiaodong Jiang; Zein-Eddine Meziani; Zhengwei Chai; Wang Xu

2001-01-01

We present measurements of the recoil proton polarization for the d(polarized y, polarized p)n reaction at thetac.m. = 90 degrees for photon energies up to 2.4 GeV. These are the first data in this reaction for polarization transfer with circularly polarized photons. The induced polarization py vanishes above 1 GeV, contrary to meson-baryon model expectations, in which resonances lead to large polarizations. However, the polarization transfer Cx does not vanish above 1 GeV, inconsistent with hadron helicity conservation. Thus, we show that the scaling behavior observed in the d(y,p)n cross sections is not a result of perturbative QCD. These data should provide important tests of new nonperturbative calculations in the intermediate energy regime

THREE-DIMENSIONAL RADIATIVE TRANSFER MODELING OF THE POLARIZATION OF THE SUN'S CONTINUOUS SPECTRUM

International Nuclear Information System (INIS)

Bueno, Javier Trujillo; Shchukina, Nataliya

2009-01-01

Polarized light provides the most reliable source of information at our disposal for diagnosing the physical properties of astrophysical plasmas, including the three-dimensional (3D) structure of the solar atmosphere. Here we formulate and solve the 3D radiative transfer problem of the linear polarization of the solar continuous radiation, which is principally produced by Rayleigh and Thomson scattering. Our approach takes into account not only the anisotropy of the solar continuum radiation but also the symmetry-breaking effects caused by the horizontal atmospheric inhomogeneities produced by the solar surface convection. We show that such symmetry-breaking effects do produce observable signatures in Q/I and U/I, even at the very center of the solar disk where we observe the forward scattering case, but their detection would require obtaining very high resolution linear polarization images of the solar surface. Without spatial and/or temporal resolution U/I ∼ 0 and the only observable quantity is Q/I, whose wavelength variation at a solar disk position close to the limb has been recently determined semi-empirically. Interestingly, our 3D radiative transfer modeling of the polarization of the Sun's continuous spectrum in a well-known 3D hydrodynamical model of the solar photosphere shows remarkable agreement with the semi-empirical determination, significantly better than that obtained via the use of one-dimensional (1D) atmospheric models. Although this result confirms that the above-mentioned 3D model was indeed a suitable choice for our Hanle-effect estimation of the substantial amount of 'hidden' magnetic energy that is stored in the quiet solar photosphere, we have found however some small discrepancies whose origin may be due to uncertainties in the semi-empirical data and/or in the thermal and density structure of the 3D model. For this reason, we have paid some attention also to other (more familiar) observables, like the center-limb variation of the

Polarized electrode enhances biological direct interspecies electron transfer for methane production in upflow anaerobic bioelectrochemical reactor.

Science.gov (United States)

Feng, Qing; Song, Young-Chae; Yoo, Kyuseon; Kuppanan, Nanthakumar; Subudhi, Sanjukta; Lal, Banwari

2018-08-01

The influence of polarized electrodes on the methane production, which depends on the sludge concentration, was investigated in upflow anaerobic bioelectrochemical (UABE) reactor. When the polarized electrode was placed in the bottom zone with a high sludge concentration, the methane production was 5.34 L/L.d, which was 53% higher than upflow anaerobic sludge blanket (UASB) reactor. However, the methane production was reduced to 4.34 L/L.d by placing the electrode in the upper zone of the UABE reactor with lower sludge concentration. In the UABE reactor, the methane production was mainly improved by the enhanced biological direct interspecies electron transfer (bDIET) pathway, and the methane production via the electrode was a minor fraction of less than 4% of total methane production. The polarized electrodes that placed in the bottom zone with a high sludge concentration enhance the bDIET for methane production in the UABE reactor and greatly improve the methane production. Copyright © 2018. Published by Elsevier Ltd.

Comparison of full-sky polarization and radiance observations to radiative transfer simulations which employ AERONET products.

Science.gov (United States)

Pust, Nathan J; Dahlberg, Andrew R; Thomas, Michael J; Shaw, Joseph A

2011-09-12

Visible-band and near infrared polarization and radiance images measured with a ground-based full-sky polarimeter are compared against a successive orders of scattering (SOS) radiative transfer model for 2009 summer cloud-free days in Bozeman, Montana, USA. The polarimeter measures radiance and polarization in 10-nm bands centered at 450 nm, 490 nm, 530 nm, 630 nm, and 700 nm. AERONET products are used to represent aerosols in the SOS model, while MISR satellite BRF products are used for the surface reflectance. While model results generally agree well with observation, the simulated degree of polarization is typically higher than observed data. Potential sources of this difference may include cloud contamination and/or underestimation of the AERONET-retrieved aerosol real refractive index. Problems with the retrieved parameters are not unexpected given the low aerosol optical depth range (0.025 to 0.17 at 500 nm) during the study and the corresponding difficulties that these conditions pose to the AERONET inversion algorithm.

Charge-Transfer States in Organic Solar Cells: Understanding the Impact of Polarization, Delocalization, and Disorder

KAUST Repository

Zheng, Zilong

2017-05-08

We investigate the impact of electronic polarization, charge delocalization, and energetic disorder on the charge-transfer (CT) states formed at a planar C60/pentacene interface. The ability to examine large complexes containing up to seven pentacene molecules and three C60 molecules allows us to take explicitly into account the electronic polarization effects. These complexes are extracted from a bilayer architecture modeled by molecular dynamics simulations and evaluated by means of electronic-structure calculations based on long-range-separated functionals (ωB97XD and BNL) with optimized range-separation parameters. The energies of the lowest charge-transfer states derived for the large complexes are in very good agreement with the experimentally reported values. The average singlet-triplet energy splittings of the lowest CT states are calculated not to exceed 10 meV. The rates of geminate recombination as well as of dissociation of the triplet excitons are also evaluated. In line with experiment, our results indicate that the pentacene triplet excitons generated through singlet fission can dissociate into separated charges on a picosecond time scale, despite the fact that their energy in C60/pentacene heterojunctions is slightly lower than the energies of the lowest CT triplet states.

The representation of neutron polarization

International Nuclear Information System (INIS)

Byrne, J.

1979-01-01

Neutron beam polarization representation is discussed under the headings; transfer matrices, coherent parity violation for neutrons, neutron spin rotation in helical magnetic fields, polarization and interference. (UK)

Some issues related to polarized radiative transfer in a multilayer medium with a changing index of refraction

International Nuclear Information System (INIS)

Garcia, R D M

2012-01-01

A couple of issues raised in a recent work on Fresnel boundary and interface conditions for polarized radiative transfer are discussed. The first issue concerns a normalization that has to be performed on the transmission matrix relating the transmitted and incident Stokes vectors at a smooth interface between different materials. It was found that the normalization step is not performed in a correct way in many existing works and so the effects of the two most frequent discrepancies encountered in these works are evaluated for a simple model of an atmosphere-water system. The second issue has to do with a choice of the sign of the parallel component of the amplitude coefficient of reflection R l when constructing the reflection matrix that relates the reflected and incident Stokes vectors at a smooth interface. A computational approach based on the limit to the case with constant index of refraction is used to determine the appropriate sign of R l for polarized radiative transfer calculations in multilayers with different indices of refraction.

Polarized and persistent Ca²⁺ plumes define loci for formation of wall ingrowth papillae in transfer cells.

Science.gov (United States)

Zhang, Hui-Ming; Imtiaz, Mohammad S; Laver, Derek R; McCurdy, David W; Offler, Christina E; van Helden, Dirk F; Patrick, John W

2015-03-01

Transfer cell morphology is characterized by a polarized ingrowth wall comprising a uniform wall upon which wall ingrowth papillae develop at right angles into the cytoplasm. The hypothesis that positional information directing construction of wall ingrowth papillae is mediated by Ca(2+) signals generated by spatiotemporal alterations in cytosolic Ca(2+) ([Ca(2+)]cyt) of cells trans-differentiating to a transfer cell morphology was tested. This hypothesis was examined using Vicia faba cotyledons. On transferring cotyledons to culture, their adaxial epidermal cells synchronously trans-differentiate to epidermal transfer cells. A polarized and persistent Ca(2+) signal, generated during epidermal cell trans-differentiation, was found to co-localize with the site of ingrowth wall formation. Dampening Ca(2+) signal intensity, by withdrawing extracellular Ca(2+) or blocking Ca(2+) channel activity, inhibited formation of wall ingrowth papillae. Maintenance of Ca(2+) signal polarity and persistence depended upon a rapid turnover (minutes) of cytosolic Ca(2+) by co-operative functioning of plasma membrane Ca(2+)-permeable channels and Ca(2+)-ATPases. Viewed paradermally, and proximal to the cytosol-plasma membrane interface, the Ca(2+) signal was organized into discrete patches that aligned spatially with clusters of Ca(2+)-permeable channels. Mathematical modelling demonstrated that these patches of cytosolic Ca(2+) were consistent with inward-directed plumes of elevated [Ca(2+)]cyt. Plume formation depended upon an alternating distribution of Ca(2+)-permeable channels and Ca(2+)-ATPase clusters. On further inward diffusion, the Ca(2+) plumes coalesced into a uniform Ca(2+) signal. Blocking or dispersing the Ca(2+) plumes inhibited deposition of wall ingrowth papillae, while uniform wall formation remained unaltered. A working model envisages that cytosolic Ca(2+) plumes define the loci at which wall ingrowth papillae are deposited. © The Author 2014. Published by Oxford

PRELIMINARY IMPEDANCE BUDGET FOR NSLS-II STORAGE RING.

Energy Technology Data Exchange (ETDEWEB)

BLEDNYKH,A.; KRINSKY, S.

2007-06-25

The wakefield and impedance produced by the components of the NSLS-II storage ring have been computed for an electron bunch length of 3mm rms. The results are summarized in a table giving for each component, the loss factor ({kappa}{sub {parallel}}), the imaginary part of the longitudinal impedance at low frequency divided by the revolution harmonic (ImZ{sub {parallel}}/n), and the transverse kick factors ({kappa}{sub x}, {kappa}{sub y}).

$\\Lambda$ and $\\bar{\\Lambda}$ polarization at COMPASS

CERN Document Server

Kang, Donghee

2010-01-01

At the COMPASS experiment $\\Lambda$ and $\\bar{\\Lambda}$ particles are produced with high statistics in deep inelastic scattering (DIS) processes of 160 GeV/c polarized muons. Since both, beam and target, are polarized, various studies on the $\\Lambda$ polarization are possible. We present results on the longitudinal polarization transfer from muons to $\\Lambda$ hyperons produced by scattering off an unpolarized isoscalar target and preliminary results on the transverse $\\Lambda$ polarization with a transversely polarized proton target. The $\\Lambda$ and $\\bar{\\Lambda}$ polarization can be studied by measuring the acceptance corrected angular distribution of its decay products. The longitudinal spin transfers to $\\Lambda$ and $\\bar{\\Lambda}$ produced in the current fragmentation region exhibit different behaviours as a function of $x_{Bj}$ and $x_{F}$. The $x_{Bj}$ and $x_{F}$ dependences of $\\Lambda$ polarization are compatible with zero, while $\\bar{\\Lambda}$ polarization tends to increase with $x_{F}$. Info...

Polarization-based enhancement of ocean color signal for estimating suspended particulate matter: radiative transfer simulations and laboratory measurements.

Science.gov (United States)

Liu, Jia; He, Xianqiang; Liu, Jiahang; Bai, Yan; Wang, Difeng; Chen, Tieqiao; Wang, Yihao; Zhu, Feng

2017-04-17

Absorption and scattering by molecules, aerosols and hydrosols, and the reflection and transmission over the sea surface can modify the original polarization state of sunlight. However, water-leaving radiance polarization, containing embedded water constituent information, has largely been neglected. Here, the efficiency of the parallel polarization radiance (PPR) for enhancing ocean color signal of suspended particulate matter is examined via vector radiative transfer simulations and laboratory experiments. The simulation results demonstrate that the PPR has a slightly higher ocean color signal at the top-of-atmosphere as compared with that of the total radiance. Moreover, both the simulations and laboratory measurements reveal that, compared with total radiance, PPR can effectively enhance the normalized ocean color signal for a large range of observation geometries, wavelengths, and suspended particle concentrations. Thus, PPR has great potential for improving the ocean color signal detection from satellite.

Improved results for the 2H(d, n)3He transverse vector polarization-transfer coefficient Kyy'(0o) at low energies

International Nuclear Information System (INIS)

Roper, C.D.; Dunham, J.D.; Clegg, T.B.; Mendez, A.J.; Tornow, W.; Walter, R.L.

2010-01-01

Measurements of the 2 H(d, n) 3 He transverse vector polarization-transfer coefficient K y y' at 0 o . are reported for 29 outgoing neutron energies between 3.94 and 8.47 MeV. Our new results determine K y y' (0 o ) more accurately than previous data, especially for neutron energies below 5 MeV. Low-energy data for this reaction are important both as a high-intensity source of highly polarized neutrons for nuclear physics studies with polarized neutron beams, and as a test of the emerging theoretical descriptions of the four-body system, where recently substantial progress has been made. (author)

Exact and approximate solutions for the one-dimensional transfer of polarized radiation, and applications to X-ray pulsars

International Nuclear Information System (INIS)

Meszaros, P.; Nagel, W.; Ventura, J.

1979-11-01

Theoretical studies of the radiation from hot, strongly magnetized plasmas, as encountered in pulsars, require a knowledge of solutions to the transfer equations for polarized radiation. We present here an analytic solution of the radiative transfer equations for one-dimensional propagation across a homogeneous slab of finite depth, as well as for a semi-infinite atmosphere. Absorption, scattering and mode-exchange between the two polarizations is included, the role of this latter being crucial. A physical discussion of the solutions for certain limiting cases, and an interpretation in terms of probabilistic (quantum escape approach) arguments, fully corrobrates these solutions, and provides a better intuitive feel for the behaviour of the radiated spectra. Whereas our analytic solutions are valid for any birefringent medium (not necessarily magnetic), our numerical examples and the qualitative discussion presented refer to the particular problem of the radiation from X-ray pulsars. Large scale qualitative changes from the nonmagnetic spectra aae found, which affect both the continum and the spectral lines. (orig.) 891 WL/orig. 892 RDG

Modified compensation algorithm of lever-arm effect and flexural deformation for polar shipborne transfer alignment based on improved adaptive Kalman filter

International Nuclear Information System (INIS)

Wang, Tongda; Cheng, Jianhua; Guan, Dongxue; Kang, Yingyao; Zhang, Wei

2017-01-01

Due to the lever-arm effect and flexural deformation in the practical application of transfer alignment (TA), the TA performance is decreased. The existing polar TA algorithm only compensates a fixed lever-arm without considering the dynamic lever-arm caused by flexural deformation; traditional non-polar TA algorithms also have some limitations. Thus, the performance of existing compensation algorithms is unsatisfactory. In this paper, a modified compensation algorithm of the lever-arm effect and flexural deformation is proposed to promote the accuracy and speed of the polar TA. On the basis of a dynamic lever-arm model and a noise compensation method for flexural deformation, polar TA equations are derived in grid frames. Based on the velocity-plus-attitude matching method, the filter models of polar TA are designed. An adaptive Kalman filter (AKF) is improved to promote the robustness and accuracy of the system, and then applied to the estimation of the misalignment angles. Simulation and experiment results have demonstrated that the modified compensation algorithm based on the improved AKF for polar TA can effectively compensate the lever-arm effect and flexural deformation, and then improve the accuracy and speed of TA in the polar region. (paper)

A New Polar Transfer Alignment Algorithm with the Aid of a Star Sensor and Based on an Adaptive Unscented Kalman Filter

Directory of Open Access Journals (Sweden)

Jianhua Cheng

2017-10-01

Full Text Available Because of the harsh polar environment, the master strapdown inertial navigation system (SINS has low accuracy and the system model information becomes abnormal. In this case, existing polar transfer alignment (TA algorithms which use the measurement information provided by master SINS would lose their effectiveness. In this paper, a new polar TA algorithm with the aid of a star sensor and based on an adaptive unscented Kalman filter (AUKF is proposed to deal with the problems. Since the measurement information provided by master SINS is inaccurate, the accurate information provided by the star sensor is chosen as the measurement. With the compensation of lever-arm effect and the model of star sensor, the nonlinear navigation equations are derived. Combined with the attitude matching method, the filter models for polar TA are designed. An AUKF is introduced to solve the abnormal information of system model. Then, the AUKF is used to estimate the states of TA. Results have demonstrated that the performance of the new polar TA algorithm is better than the state-of-the-art polar TA algorithms. Therefore, the new polar TA algorithm proposed in this paper is effectively to ensure and improve the accuracy of TA in the harsh polar environment.

A New Polar Transfer Alignment Algorithm with the Aid of a Star Sensor and Based on an Adaptive Unscented Kalman Filter.

Science.gov (United States)

Cheng, Jianhua; Wang, Tongda; Wang, Lu; Wang, Zhenmin

2017-10-23

Because of the harsh polar environment, the master strapdown inertial navigation system (SINS) has low accuracy and the system model information becomes abnormal. In this case, existing polar transfer alignment (TA) algorithms which use the measurement information provided by master SINS would lose their effectiveness. In this paper, a new polar TA algorithm with the aid of a star sensor and based on an adaptive unscented Kalman filter (AUKF) is proposed to deal with the problems. Since the measurement information provided by master SINS is inaccurate, the accurate information provided by the star sensor is chosen as the measurement. With the compensation of lever-arm effect and the model of star sensor, the nonlinear navigation equations are derived. Combined with the attitude matching method, the filter models for polar TA are designed. An AUKF is introduced to solve the abnormal information of system model. Then, the AUKF is used to estimate the states of TA. Results have demonstrated that the performance of the new polar TA algorithm is better than the state-of-the-art polar TA algorithms. Therefore, the new polar TA algorithm proposed in this paper is effectively to ensure and improve the accuracy of TA in the harsh polar environment.

Reduction of coating induced polarization aberrations by controlling the polarization state variation

International Nuclear Information System (INIS)

Li, Yanghui; Shen, Weidong; Zheng, Zhenrong; Zhang, Yueguang; Liu, Xu; Hao, Xiang

2011-01-01

The mechanism of coating induced polarization state variation is analysed by the Jones matrix. Pauli spin matrices are used to establish the relationship between coating induced polarization state variation and polarization aberrations. To reduce coating induced polarization aberrations, we propose that δ = 0 and T s = T p at arbitrary incident angle should be appended as two additional optimization goals of optical coating design when the requirements of transmittance are met. Two typical anti-reflection (AR) coatings are designed and the polarization state variation induced by them is simulated. The MTF (modulation transfer function) calculated by polarization ray tracing is applied to evaluate the polarization aberrations of the practical lithography objective system with the two AR coatings. All the obtained results show that the coating induced polarization aberrations can be reduced by optimizing the angle dependent properties of the optical coating without additional optical elements

Incorporation of charge transfer into the explicit polarization fragment method by grand canonical density functional theory.

Science.gov (United States)

Isegawa, Miho; Gao, Jiali; Truhlar, Donald G

2011-08-28

Molecular fragmentation algorithms provide a powerful approach to extending electronic structure methods to very large systems. Here we present a method for including charge transfer between molecular fragments in the explicit polarization (X-Pol) fragment method for calculating potential energy surfaces. In the conventional X-Pol method, the total charge of each fragment is preserved, and charge transfer between fragments is not allowed. The description of charge transfer is made possible by treating each fragment as an open system with respect to the number of electrons. To achieve this, we applied Mermin's finite temperature method to the X-Pol wave function. In the application of this method to X-Pol, the fragments are open systems that partially equilibrate their number of electrons through a quasithermodynamics electron reservoir. The number of electrons in a given fragment can take a fractional value, and the electrons of each fragment obey the Fermi-Dirac distribution. The equilibrium state for the electrons is determined by electronegativity equalization with conservation of the total number of electrons. The amount of charge transfer is controlled by re-interpreting the temperature parameter in the Fermi-Dirac distribution function as a coupling strength parameter. We determined this coupling parameter so as to reproduce the charge transfer energy obtained by block localized energy decomposition analysis. We apply the new method to ten systems, and we show that it can yield reasonable approximations to potential energy profiles, to charge transfer stabilization energies, and to the direction and amount of charge transferred. © 2011 American Institute of Physics

Photoinduced Electron Transfer of PAMAM Dendrimer-Zinc(II) Porphyrin Associates at Polarized Liquid|Liquid Interfaces.

Science.gov (United States)

Nagatani, Hirohisa; Sakae, Hiroki; Torikai, Taishi; Sagara, Takamasa; Imura, Hisanori

2015-06-09

The heterogeneous photoinduced electron-transfer reaction of the ion associates between NH2-terminated polyamidoamine (PAMAM) dendrimers and 5,10,15,20-tetrakis(4-sulfonatophenyl)porphyrinato zinc(II) (ZnTPPS(4-)) was studied at the polarized water|1,2-dichloroethane (DCE) interface. The positive photocurrent arising from the photoreduction of ZnTPPS(4-) by a lipophilic quencher, decamethylferrocene, in the interfacial region was significantly enhanced by the ion association with the PAMAM dendrimers. The photocurrent response of the dendrimer-ZnTPPS(4-) associates was dependent on the pH condition and on the generation of dendrimer. A few cationic additives such as polyallylamine and n-octyltrimethyammonium were also examined as alternatives to the PAMAM dendrimer, but the magnitude of the photocurrent enhancement was rather small. The high photoreactivity of the dendrimer-ZnTPPS(4-) associates was interpreted mainly as a result of the high interfacial concentration of photoreactive porphyrin units associated stably with the dendrimer which was preferably adsorbed at the polarized water|DCE interface. The photochemical data observed in the second and fourth generation PAMAM dendrimer systems demonstrated that the higher generation dendrimer which can incorporate a porphyrin molecule more completely in the interior is less efficient for the photocurrent enhancement at the interface. These results indicated that the photoreactivity of ionic reactant at a polarized liquid|liquid interface can readily be modified via ion association with the charged dendrimer.

Improved Results for the H-2(d, n)(3) He Transverse Vector Polarization- Transfer Coefficient K-y(y)' (0 degrees) at Low Energies

International Nuclear Information System (INIS)

Roper, C.D.; Clegg, T.; Dunham, J.D.; Mendez, Anthony J. II; Tornow, W.; Walter, R.L.

2010-01-01

Measurements of the H-2(d, n)(3) He transverse vector polarization-transfer coefficient K-y(y)' at 0 degrees. are reported for 29 outgoing neutron energies between 3.94 and 8.47MeV. Our new results determine K-y(y)' (0 degrees) more accurately than previous data, especially for neutron energies below 5MeV. Low-energy data for this reaction are important both as a high-intensity source of highly polarized neutrons for nuclear physics studies with polarized neutron beams, and as a test of the emerging theoretical descriptions of the four-body system, where recently substantial progress has been made.

Measurement of polarization-transfer to bound protons in carbon and its virtuality dependence

Science.gov (United States)

Izraeli, D.; Brecelj, T.; Achenbach, P.; Ashkenazi, A.; Böhm, R.; Cohen, E. O.; Distler, M. O.; Esser, A.; Gilman, R.; Kolar, T.; Korover, I.; Lichtenstadt, J.; Mardor, I.; Merkel, H.; Mihovilovič, M.; Müller, U.; Olivenboim, M.; Piasetzky, E.; Ron, G.; Schlimme, B. S.; Schoth, M.; Sfienti, C.; Širca, S.; Štajner, S.; Strauch, S.; Thiel, M.; Weber, A.; Yaron, I.; A1 Collaboration

2018-06-01

We measured the ratio Px /Pz of the transverse to longitudinal components of polarization transferred from electrons to bound protons in 12C by the 12C (e → ,e‧ p →) process at the Mainz Microtron (MAMI). We observed consistent deviations from unity of this ratio normalized to the free-proton ratio, (Px /Pz) 12C /(Px /Pz) 1H, for both s- and p-shell knocked out protons, even though they are embedded in averaged local densities that differ by about a factor of two. The dependence of the double ratio on proton virtuality is similar to the one for knocked out protons from 2H and 4He, suggesting a universal behavior. It further implies no dependence on average local nuclear density.

Measurement of the polarization parameter in 24 GeV/c pp elastic scattering at large momentum transfers

CERN Document Server

Antille, J; Dick, Louis; Gonidec, A; Kuroda, K; Kyberd, P; Michalowicz, A; Perret-Gallix, D; Salmon, G L; Werlen, M

1981-01-01

A measurement of the polarization parameter P/sub 0/ in pp elastic scattering has been made 24 GeV/c over the range of momentum transfer squared 0.7< mod t mod <5.0 (GeV/c)/sup 2/. The structure of P/sub 0/ has changed compared to typical lower energy data. The second peak is suppressed and a dip has appeared at mod t mod =3.6 (GeV/c)/sup 2/. (31 refs).

Comparison of discrete ordinate and Monte Carlo simulations of polarized radiative transfer in two coupled slabs with different refractive indices.

Science.gov (United States)

Cohen, D; Stamnes, S; Tanikawa, T; Sommersten, E R; Stamnes, J J; Lotsberg, J K; Stamnes, K

2013-04-22

A comparison is presented of two different methods for polarized radiative transfer in coupled media consisting of two adjacent slabs with different refractive indices, each slab being a stratified medium with no change in optical properties except in the direction of stratification. One of the methods is based on solving the integro-differential radiative transfer equation for the two coupled slabs using the discrete ordinate approximation. The other method is based on probabilistic and statistical concepts and simulates the propagation of polarized light using the Monte Carlo approach. The emphasis is on non-Rayleigh scattering for particles in the Mie regime. Comparisons with benchmark results available for a slab with constant refractive index show that both methods reproduce these benchmark results when the refractive index is set to be the same in the two slabs. Computed results for test cases with coupling (different refractive indices in the two slabs) show that the two methods produce essentially identical results for identical input in terms of absorption and scattering coefficients and scattering phase matrices.

Design of a tensor polarized deuterium target polarized by spin-exchange with optically pumped NA

International Nuclear Information System (INIS)

Green, M.C.

1984-01-01

A proposed design for a tensor polarized deuterium target (approx. 10 15 atoms/cm 2 ) for nuclear physics studies in an electron storage ring accelerator is presented. The deuterium atoms undergo electron spin exchange with a highly polarized sodium vapor; this polarization is transferred to the deuterium nuclei via the hyperfine interaction. The deuterium nuclei obtain their tensor polarization through repeated electron spin exchange/hyperfine interactions. The sodium vapor polarization is maintained by standard optical pumping techniques. Model calculations are presented in detail leading to a discussion of the expected performance and the technical obstacles to be surmounted in the development of such a target

Design of a tensor polarized deuterium target polarized by spin-exchange with optically pumped NA

International Nuclear Information System (INIS)

Green, M.C.

1984-05-01

A proposed design for a tensor polarized deuterium target (approx. 10 15 atoms/cm 2 ) for nuclear physics studies in an electron storage ring accelerator is presented. The deuterium atoms undergo electron spin exchange with a highly polarized sodium vapor; this polarization is transferred to the deuterium nuclei via the hyperfine interaction. The deuterium nuclei obtain their tensor polarization through repeated electron spin exchange/hyperfine interactions. The sodium vapor polarization is maintained by standard optical pumping techniques. Model calculations are presented in detail leading to a discussion of the expected performance and the technical obstacles to be surmounted in the development of such a target. 15 references, 10 figures

The polar 2e/12c bond in phenalenyl-azaphenalenyl hetero-dimers: Stronger stacking interaction and fascinating interlayer charge transfer

Energy Technology Data Exchange (ETDEWEB)

Zhong, Rong-Lin; Li, Zhi-Ru, E-mail: hlxu@nenu.edu.cn, E-mail: lzr@jlu.edu.cn [Institute of Theoretical Chemistry, Jilin University, Changchun 130023 (China); Xu, Hong-Liang, E-mail: hlxu@nenu.edu.cn, E-mail: lzr@jlu.edu.cn [Institute of Functional Material Chemistry, Faculty of Chemistry, Northeast Normal University, Changchun, Jilin 130024 (China)

2016-08-07

An increasing number of chemists have focused on the two-electron/multicenter bond (2e/mc) that was first introduced to interpret the bonding mechanism of radical dimers. Herein, we report the polar two-electron/twelve center (2e/12c) bonding character in a series of phenalenyl-azaphenalenyl radical hetero-dimers. Interestingly, the bonding energy of weaker polar hetero-dimer (P-TAP) is dominated by the overlap of the two different singly occupied molecular orbital of radicals, while that of stronger polar hetero-dimer (P-HAP) is dominated by the electrostatic attraction. Results show that the difference between the electronegativity of the monomers plays a prominent role in the essential attribution of the polar 2e/12c bond. Correspondingly, a stronger stacking interaction in the hetero-dimer could be effectively achieved by increasing the difference of nitrogen atoms number between the monomers. It is worthy of note that an interesting interlayer charge transfer character is induced in the polar hetero-dimers, which is dependent on the difference between the electronegativity of the monomers. It is our expectation that the new knowledge about the bonding nature of radical hetero-dimers might provide important information for designing radical based functional materials with various applications.

Feasibility studies of a polarized positron source based on the Bremsstrahlung of polarized electrons

International Nuclear Information System (INIS)

Dumas, J.

2011-09-01

The nuclear and high-energy physics communities have shown a growing interest in the availability of high current, highly-polarized positron beams. A sufficiently energetic polarized photon or lepton incident on a target may generate, via Bremsstrahlung and pair creation within a solid target foil, electron-positron pairs that should carry some fraction of the initial polarization. Recent advances in high current (> 1 mA) spin polarized electron sources at Jefferson Lab offer the perspective of creating polarized positrons from a low energy electron beam. This thesis discusses polarization transfer from electrons to positrons in the perspective of the design optimization of a polarized positron source. The PEPPo experiment, aiming at a measurement of the positron polarization from a low energy (< 10 MeV) highly spin polarized electron beam is discussed. A successful demonstration of this technique would provide an alternative scheme for the production of low energy polarized positrons and useful information for the optimization of the design of polarized positron sources in the sub-GeV energy range. (author)

Markov chain formalism for generalized radiative transfer in a plane-parallel medium, accounting for polarization

International Nuclear Information System (INIS)

Xu, Feng; Davis, Anthony B.; Diner, David J.

2016-01-01

A Markov chain formalism is developed for computing the transport of polarized radiation according to Generalized Radiative Transfer (GRT) theory, which was developed recently to account for unresolved random fluctuations of scattering particle density and can also be applied to unresolved spectral variability of gaseous absorption as an improvement over the standard correlated-k method. Using Gamma distribution to describe the probability density function of the extinction or absorption coefficient, a shape parameter a that quantifies the variability is introduced, defined as the mean extinction or absorption coefficient squared divided by its variance. It controls the decay rate of a power-law transmission that replaces the usual exponential Beer-Lambert-Bouguer law. Exponential transmission, hence classic RT, is recovered when a→∞. The new approach is verified to high accuracy against numerical benchmark results obtained with a custom Monte Carlo method. For a<∞, angular reciprocity is violated to a degree that increases with the spatial variability, as observed for finite portions of real-world cloudy scenes. While the degree of linear polarization in liquid water cloudbows, supernumerary bows, and glories is affected by spatial heterogeneity, the positions in scattering angle of these features are relatively unchanged. As a result, a single-scattering model based on the assumption of subpixel homogeneity can still be used to derive droplet size distributions from polarimetric measurements of extended stratocumulus clouds. - Highlights: • A Markov chain formalism is developed for Generalized Radiative Transfer theory. • Angular reciprocity is violated to a degree that increases with spatial variability. • The positions of cloudbows and glories in scattering angle are relatively unchanged.

Investigation of the NN interaction from polarization transfer experiments in low energy pp scattering

Energy Technology Data Exchange (ETDEWEB)

Weidmann, R.; Albert, J.; Glombik, A.; Kretschmer, W.; Nebert, P.; Rauscher, A. (Physikalisches Inst., Univ. Erlangen-Nuernberg (Germany)); Clajus, M.; Egun, P.M.; Grueebler, W.; Hautle, P. (Inst. fuer Mittelenergiephysik, ETH, Zurich (Switzerland)); Schmelzbach, P.A. (Paul Scherrer Inst., F1, Accelerator Div., Villigen (Switzerland)); Slaus, I. (Inst. Ruder Boscovic, Zagreb (Croatia))

1993-03-01

The polarization-Transfer observables K[sub y][sup y']([theta]), K[sub x][sup x']([theta]) and K[sub z][sup x']([theta]) for proton-proton scattering have been measured at E[sub p]=25.68 MeV. A simultaneous phase-shift analysis of these new data with differential cross section and analyzing power data at the same energy resulted in a very accurate determination of the p-wave phase-shift combinations [Delta][sub C], [Delta][sub LS] and [Delta][sub T] and of the [sup 3]F[sub 2]-[sup 3]P[sub 2] mixing parameter [epsilon][sub 2]. With this complete set of high precision data a critical test of microscopic NN-potential models has been performed. (orig.).

Single Transition-to-single Transition Polarization Transfer (ST2-PT) in [15N,1H]-TROSY

International Nuclear Information System (INIS)

Pervushin, Konstantin V.; Wider, Gerhard; Wuethrich, Kurt

1998-01-01

This paper describes the use of single transition-to-single transition polarization transfer (ST2-PT) in transverse relaxation-optimized spectroscopy (TROSY), where it affords a √2 sensitivity enhancement for kinetically stable amide 15N-1H groups in proteins. Additional, conventional improvements of [15N,1H]-TROSY include that signal loss for kinetically labile 15N-1H groups due to saturation transfer from the solvent water is suppressed with the 'water flip back' technique and that the number of phase steps is reduced to two, which is attractive for the use of [15N,1H]-TROSY as an element in more complex NMR schemes. Finally, we show that the impact of the inclusion of the 15N steady-state magnetization (Pervushin et al., 1998) on the signal-to-noise ratio achieved with [15N,1H]-TROSY exceeds by up to two-fold the gain expected from the gyromagnetic ratios of 1H and 15N

Transfer of polarized light in planetary atmospheres basic concepts and practical methods

CERN Document Server

Hovenier, Joop W; Domke, Helmut

2004-01-01

The principal elements of the theory of polarized light transfer in planetary atmospheres are expounded in a systematic but concise way. Basic concepts and practical methods are emphasized, both for single and multiple scattering of electromagnetic radiation by molecules and particles in the atmospheres of planets in the Solar System, including the Earth, and beyond. A large part of the book is also useful for studies of light scattering by particles in comets, the interplanetary and interstellar medium, circumstellar disks, reflection nebulae, water bodies like oceans and suspensions of particles in a gas or liquid in the laboratory. Throughout the book symmetry principles, such as the reciprocity principle and the mirror symmetry principle, are employed. In this way the theory is made more transparent and easier to understand than in most papers on the subject. In addition, significant computational reductions, resulting from symmetry principles, are presented. Hundreds of references to relevant literature ...

Zero-field spin transfer oscillators based on magnetic tunnel junction having perpendicular polarizer and planar free layer

Directory of Open Access Journals (Sweden)

Bin Fang

2016-12-01

Full Text Available We experimentally studied spin-transfer-torque induced magnetization oscillations in an asymmetric MgO-based magnetic tunnel junction device consisting of an in-plane magnetized free layer and an out-of-plane magnetized polarizer. A steady auto-oscillation was achieved at zero magnetic field and room temperature, with an oscillation frequency that was strongly dependent on bias currents, with a large frequency tunability of 1.39 GHz/mA. Our results suggest that this new structure has a high potential for new microwave device designs.

Achievement of transportable polarized D, in solid HD, with a one day passively maintained polarization

International Nuclear Information System (INIS)

Honig, A.; Alexander, N.; Fan, Q.; Wei, X.; Yu, Y.Y.

1993-01-01

At a previous workshop, we discussed evaporating solid HD with spin-polarized deuterons to produce a high density polarized deuteron gaseous internal target. Since then, we have achieved in solid HD 38% polarized D, whose spin-lattice relaxation time at 1.5 K in a field of 0.1 T is of the order of a day. Optimization of the procedure with the present apparatus should result in 60% D polarization, and longer polarization holding times. The polarized sample of approximately 0.2 cm 3 volume used here is extractable from the dilution refrigerator with a cold-transfer apparatus which maintains the sample at or below 5 K, insuring retention of the high polarization. It is subsequently insertable into a variety of systems, and employable as a polarized solid, liquid, or gas. We are exploring the possibility of extending the polarization maintenance time to about a month (with a matched 1 month preparation time), of polarizing metastably H as well as D, and of producing much larger samples, of the order of 100 cm 3

Observer variation in FDG PET-CT for staging of non-small-cell lung carcinoma

Energy Technology Data Exchange (ETDEWEB)

Hofman, Michael S. [St Thomas' Hospital, PET Imaging Centre, London (United Kingdom)]|[Southern Health, Nuclear Medicine, Melbourne (Australia); Smeeton, Nigel C. [King' s College London, Division of Health and Social Care Research, London (United Kingdom); Rankin, Sheila C.; Nunan, Tom; O' Doherty, Michael J. [St Thomas' Hospital, PET Imaging Centre, London (United Kingdom)

2009-02-15

Error and variation in reporting remains one of the weakest features of clinical imaging despite enormous technological advances in nuclear medicine and radiology. The aim of this study was to evaluate agreement amongst experienced readers in staging non-small-cell lung cancer (NSCLC) with PET-CT. A series of {sup 18}F-FDG PET-CT scans from 100 consecutive patients were reviewed independently by three experienced readers, with two readers reviewing each scan series a second time. Individual mediastinal lymph node stations were assessed as benign/inflammatory, equivocal or malignant, and AJCC N and M stage were also assigned. Kappa ({kappa}) was used to compare ratings from two categories and weighted kappa ({kappa}{sub w}) for three or more categories, and kappa values were interpreted according to the Landis-Koch benchmarks. Both intra- and interobserver agreement for N and M staging were high. For M staging there was almost perfect intra- and interobserver agreement ({kappa} = 0.90-0.93). For N staging, agreement was either almost perfect or substantial (intraobserver {kappa}{sub w} = 0.79, 0.91; interobserver {kappa}{sub w} = 0.75-0.81). Importantly, there was almost perfect agreement for N0/1 vs N2/3 disease ({kappa} = 0.80-0.97). Agreement for inferior and superior mediastinal nodes (stations 1, 2, 3, 7, 8, 9) was either almost perfect or substantial ({kappa}{sub w} = 0.71-0.88), but lower for hilar nodes (10; {kappa}{sub w} = 0.56-0.71). Interreporter variability was greatest for aortopulmonary nodes (5, 6; {kappa}{sub w} = 0.48-0.55). Amongst experienced reporters in a single centre, there was a very high level of agreement for both mediastinal nodal stage and detection of distant metastases with PET-CT. This supports the use of PET-CT as a robust imaging modality for staging NSCLC. (orig.)

POLARIZED LINE FORMATION WITH LOWER-LEVEL POLARIZATION AND PARTIAL FREQUENCY REDISTRIBUTION

Energy Technology Data Exchange (ETDEWEB)

Supriya, H. D.; Sampoorna, M.; Nagendra, K. N.; Ravindra, B. [Indian Institute of Astrophysics, Bangalore 560034 (India); Stenflo, J. O. [Institute of Astronomy, ETH Zurich, CH-8093 Zurich (Switzerland)

2016-09-10

In the well-established theories of polarized line formation with partial frequency redistribution (PRD) for a two-level and two-term atom, it is generally assumed that the lower level of the scattering transition is unpolarized. However, the existence of unexplained spectral features in some lines of the Second Solar Spectrum points toward a need to relax this assumption. There exists a density matrix theory that accounts for the polarization of all the atomic levels, but it is based on the flat-spectrum approximation (corresponding to complete frequency redistribution). In the present paper we propose a numerical algorithm to solve the problem of polarized line formation in magnetized media, which includes both the effects of PRD and the lower level polarization (LLP) for a two-level atom. First we derive a collisionless redistribution matrix that includes the combined effects of the PRD and the LLP. We then solve the relevant transfer equation using a two-stage approach. For illustration purposes, we consider two case studies in the non-magnetic regime, namely, the J {sub a} = 1, J {sub b} = 0 and J {sub a} = J {sub b} = 1, where J {sub a} and J {sub b} represent the total angular momentum quantum numbers of the lower and upper states, respectively. Our studies show that the effects of LLP are significant only in the line core. This leads us to propose a simplified numerical approach to solve the concerned radiative transfer problem.

The Transfer of Resonance Line Polarization with Partial Frequency Redistribution in the General Hanle–Zeeman Regime

Energy Technology Data Exchange (ETDEWEB)

Ballester, E. Alsina; Bueno, J. Trujillo [Instituto de Astrofísica de Canarias, E-38205 La Laguna, Tenerife (Spain); Belluzzi, L., E-mail: ealsina@iac.es [Istituto Ricerche Solari Locarno, CH-6605 Locarno Monti (Switzerland)

2017-02-10

The spectral line polarization encodes a wealth of information about the thermal and magnetic properties of the solar atmosphere. Modeling the Stokes profiles of strong resonance lines is, however, a complex problem both from a theoretical and computational point of view, especially when partial frequency redistribution (PRD) effects need to be taken into account. In this work, we consider a two-level atom in the presence of magnetic fields of arbitrary intensity (Hanle–Zeeman regime) and orientation, both deterministic and micro-structured. Working within the framework of a rigorous PRD theoretical approach, we have developed a numerical code that solves the full non-LTE radiative transfer problem for polarized radiation, in one-dimensional models of the solar atmosphere, accounting for the combined action of the Hanle and Zeeman effects, as well as for PRD phenomena. After briefly discussing the relevant equations, we describe the iterative method of solution of the problem and the numerical tools that we have developed and implemented. We finally present some illustrative applications to two resonance lines that form at different heights in the solar atmosphere, and provide a detailed physical interpretation of the calculated Stokes profiles. We find that magneto-optical effects have a strong impact on the linear polarization signals that PRD effects produce in the wings of strong resonance lines. We also show that the weak-field approximation has to be used with caution when PRD effects are considered.

Development of Efficient and Robust Heteronuclear Cross-Polarization Techniques for Biological Solid-State Nuclear Magnetic Resonance Spectroscopy

DEFF Research Database (Denmark)

Jain, Sheetal Kumar

2014-01-01

→13C and 1H→14N polarization transfers. The deuterium experiments were performed on deuterated glutamine and outer membrane protein G samples, while the nitrogen experiments were carried out on ammonium nitrate and alanine samples. Moreover, experiments with low power on the 2H channel are presented......→13C polarization transfer to facilitate 2-dimensional experiments detecting 14N in the indirect dimension are shown. Finally, to test the polarization transfer efficiency with very large chemical shift anisotropies, 19F→13C polarization transfer experiments for Poly Tetra Fluoro Ethylene (PTFE...

Radiative transfer in atmosphere-sea ice-ocean system

Energy Technology Data Exchange (ETDEWEB)

Jin, Z.; Stamnes, K.; Weeks, W.F. [Univ. of Alaska, Fairbanks, AK (United States); Tsay, S.C. [NASA Goddard Space Flight Center, Greenbelt, MD (United States)

1996-04-01

Radiative energy is critical in controlling the heat and mass balance of sea ice, which significantly affects the polar climate. In the polar oceans, light transmission through the atmosphere and sea ice is essential to the growth of plankton and algae and, consequently, to the microbial community both in the ice and in the ocean. Therefore, the study of radiative transfer in the polar atmosphere, sea ice, and ocean system is of particular importance. Lacking a properly coupled radiative transfer model for the atmosphere-sea ice-ocean system, a consistent study of the radiative transfer in the polar atmosphere, snow, sea ice, and ocean system has not been undertaken before. The radiative transfer processes in the atmosphere and in the ice and ocean have been treated separately. Because the radiation processes in the atmosphere, sea ice, and ocean depend on each other, this separate treatment is inconsistent. To study the radiative interaction between the atmosphere, clouds, snow, sea ice, and ocean, a radiative transfer model with consistent treatment of radiation in the coupled system is needed and is under development.

CpG Oligodeoxynucleotides Enhance the Efficacy of Adoptive Cell Transfer Using Tumor Infiltrating Lymphocytes by Modifying the Th1 Polarization and Local Infiltration of Th17 Cells

Directory of Open Access Journals (Sweden)

Lin Xu

2010-01-01

Full Text Available Adoptive cell transfer immunotherapy using tumor infiltrating lymphocytes (TILs was an important therapeutic strategy against tumors. But the efficacy remains limited and development of new strategies is urgent. Recent evidence suggested that CpG-ODNs might be a potent candidate for tumor immunotherapy. Here we firstly reported that CpG-ODNs could significantly enhance the antitumor efficacy of adoptively transferred TILs in vivo accompanied by enhanced activity capacity and proliferation of CD8+ T cells and CD8+ T cells, as well as a Th1 polarization immune response. Most importantly, we found that CpG-ODNs could significantly elevate the infiltration of Th17 cells in tumor mass, which contributed to anti-tumor efficacy of TILs in vivo. Our findings suggested that CpG ODNs could enhance the anti-tumor efficacy of adoptively transferred TILs through modifying Th1 polarization and local infiltration of Th17 cells, which might provide a clue for developing a new strategy for ACT based on TILs.

Radiation transfer and stellar atmospheres

Science.gov (United States)

Swihart, T. L.

This is a revised and expanded version of the author's Basic Physics of Stellar Atmospheres, published in 1971. The equation of transfer is considered, taking into account the intensity and derived quantities, the absorption coefficient, the emission coefficient, the source function, and special integrals for plane media. The gray atmosphere is discussed along with the nongray atmosphere, and aspects of line formation. Topics related to polarization are explored, giving attention to pure polarized radiation, general polarized radiation, transfer in a magnetic plasma, and Rayleigh scattering and the sunlit sky. Physical and astronomical constants, and a number of problems related to the subjects of the book are presented in an appendix.

Properties of baryonic, electric and strangeness chemical potentials and some of their consequences in relativistic heavy ion collisions

Energy Technology Data Exchange (ETDEWEB)

Mekjian, Aram Z. [Rutgers University, Department of Physics and Astronomy, Piscataway, NJ 08854 (United States) and California Institute of Technology, Kellogg Radiation Laboratory 106-38, Pasadena, CA 91125 (United States)]. E-mail: mekjian@physics.rutgers.edu

2007-07-19

Analytic expressions are given for the baryonic, electric and strangeness chemical potentials which explicitly show the importance of various terms. Simple scaling relations connecting these chemical potentials are found. Applications to particle ratios and to fluctuations and related thermal properties such as the isothermal compressibility {kappa}{sub T} are illustrated. A possible divergence of {kappa}{sub T} is discussed.

Ejectile polarization and nuclear orbitals

International Nuclear Information System (INIS)

Ohnishi, A.; Maruyama, T.; Horiuchi, H.

1992-01-01

Ejectile polarization phenomena are studied by the use of 'Quantum Molecular Dynamics plus external mean field' model. It is shown that the far-side contribution increases as the incident energy increases or the target charge decreases. The incident energy and the target dependence of ejectile polarization data is reproduced qualitatively. The near- and far-side contributions themselves are calculated to be almost monotone functions of ejectile momentum as is predicted in a simple projectile fragmentation scheme without the assumption that the linear and angular momentum transfers are negligible, and their statistical average results in various shapes in ejectile polarization

Robust techniques for polarization and detection of nuclear spin ensembles

Science.gov (United States)

Scheuer, Jochen; Schwartz, Ilai; Müller, Samuel; Chen, Qiong; Dhand, Ish; Plenio, Martin B.; Naydenov, Boris; Jelezko, Fedor

2017-11-01

Highly sensitive nuclear spin detection is crucial in many scientific areas including nuclear magnetic resonance spectroscopy, magnetic resonance imaging (MRI), and quantum computing. The tiny thermal nuclear spin polarization represents a major obstacle towards this goal which may be overcome by dynamic nuclear spin polarization (DNP) methods. The latter often rely on the transfer of the thermally polarized electron spins to nearby nuclear spins, which is limited by the Boltzmann distribution of the former. Here we utilize microwave dressed states to transfer the high (>92 % ) nonequilibrium electron spin polarization of a single nitrogen-vacancy center (NV) induced by short laser pulses to the surrounding 13C carbon nuclear spins. The NV is repeatedly repolarized optically, thus providing an effectively infinite polarization reservoir. A saturation of the polarization of the nearby nuclear spins is achieved, which is confirmed by the decay of the polarization transfer signal and shows an excellent agreement with theoretical simulations. Hereby we introduce the polarization readout by polarization inversion method as a quantitative magnetization measure of the nuclear spin bath, which allows us to observe by ensemble averaging macroscopically hidden polarization dynamics like Landau-Zener-Stückelberg oscillations. Moreover, we show that using the integrated solid effect both for single- and double-quantum transitions nuclear spin polarization can be achieved even when the static magnetic field is not aligned along the NV's crystal axis. This opens a path for the application of our DNP technique to spins in and outside of nanodiamonds, enabling their application as MRI tracers. Furthermore, the methods reported here can be applied to other solid state systems where a central electron spin is coupled to a nuclear spin bath, e.g., phosphor donors in silicon and color centers in silicon carbide.

Transfers of Colloidal Silica from Water into Organic Solvents of Intermediate Polarities

Science.gov (United States)

Kasseh; Keh

1998-01-15

Dispersions of discrete metal-oxide submicroparticles in organic solvents of medium polarities are uneasy to generate and weakly documented. We address this topic along two general methods focusing on silica. Successive transfers of colloidal particles from water into n-propanol and then into 1,2-dichloroethane by azeotropic distillation yield a stable organosol. The particles are found to be propanol-coated by surface esterification to the extent of 0.40 nm2 per molecule. Alternatively, centrifugation-redispersion cycles make it possible to obtain stable suspensions of unaltered silica in methanol and acetonitrile starting from an aqueous silicasol. Particles are characterized by various methods including nitrogen adsorption, transmission electron microscopy, dynamic light scattering, and electrophoresis. The stabilities of these suspensions in various organic solvents are investigated with special concern for the role of residual water. Stabilization of silica in methanol is inconspicuously related to solvent permittivity and prominently dependent on the presence of adsorbed water. In contrast, the acetonitrile silicasol, which is unaffected by residual water, displays electrophoretic behavior compatible with electrostatic stabilization. Copyright 1998 Academic Press. Copyright 1998Academic Press

Genetic modification of adeno-associated viral vector type 2 capsid enhances gene transfer efficiency in polarized human airway epithelial cells.

Science.gov (United States)

White, April F; Mazur, Marina; Sorscher, Eric J; Zinn, Kurt R; Ponnazhagan, Selvarangan

2008-12-01

Cystic fibrosis (CF) is a common genetic disease characterized by defects in the expression of the CF transmembrane conductance regulator (CFTR) gene. Gene therapy offers better hope for the treatment of CF. Adeno-associated viral (AAV) vectors are capable of stable expression with low immunogenicity. Despite their potential in CF gene therapy, gene transfer efficiency by AAV is limited because of pathophysiological barriers in these patients. Although a few AAV serotypes have shown better transduction compared with the AAV2-based vectors, gene transfer efficiency in human airway epithelium has still not reached therapeutic levels. To engineer better AAV vectors for enhanced gene delivery in human airway epithelium, we developed and characterized mutant AAV vectors by genetic capsid modification, modeling the well-characterized AAV2 serotype. We genetically incorporated putative high-affinity peptide ligands to human airway epithelium on the GH loop region of AAV2 capsid protein. Six independent mutant AAV were constructed, containing peptide ligands previously reported to bind with high affinity for known and unknown receptors on human airway epithelial cells. The vectors were tested on nonairway cells and nonpolarized and polarized human airway epithelial cells for enhanced infectivity. One of the mutant vectors, with the peptide sequence THALWHT, not only showed the highest transduction in undifferentiated human airway epithelial cells but also indicated significant transduction in polarized cells. Interestingly, this modified vector was also able to infect cells independently of the heparan sulfate proteoglycan receptor. Incorporation of this ligand on other AAV serotypes, which have shown improved gene transfer efficiency in the human airway epithelium, may enhance the application of AAV vectors in CF gene therapy.

The coprecipitation of Sr2+ with calcite at 250C and 1 atm

International Nuclear Information System (INIS)

Pingitore, N.E. Jr.; Eastman, M.P.

1986-01-01

The incorporation of Sr 2+ into calcite at earth surface aqueous conditions is affected by the absolute concentration of Sr 2+ , the presence of Ba 2+ and NaCl in the solution and the rate of precipitation. At solution ratios (molar) of Sr 2+ to Ca 2+ in the low 10 -3 range, which yield calcites with several hundred ppm Sr 2+ , kappasub(calcite) sup(Sr) typically assumes a value between 0.10 and 0.20. Above these concentrations the value of kappasub(calcite) sup(Sr) drops to approximately 0.06. Furthermore, if minor amounts of Ba 2+ or large amounts of Na + (0.48 M) are added to a dilute Sr 2+ solution, a value around 0.06 for kappasub(calcite)sup(Sr) is found. This 'strontium concentration effect' and the associated 'competitive cation effect' suggest that small amounts of Sr 2+ may be incorporated into a limited number of nonlattice sites in calcite. Incorporation of Sr 2+ into these sites, presumably defects, noticeably affects kappasub(calcite)sup(Sr) only at low Sr 2+ concentrations and in the absence of competition from other large cations. An increase in kappasub(calcite)sup(Sr) with rate of precipitation, qualitatively similar to that found in other studies, was observed only when precipitation times were decreased from days to hours. For many geologic settings a partition coefficient for Sr 2+ into calcite of 0.06 appears appropriate, but there are situations - very low Sr 2+ concentrations, the presence of Mg 2+ , and fast precipitation rates - in which a larger value might better approximate natural partitioning. (author)

Production of spin-polarized unstable nuclei by using polarized electron capture process

International Nuclear Information System (INIS)

Shimizu, S.

1998-01-01

Measurements of emitted radiation from spin polarized nuclei are used to get information on electromagnetic moment of ground state unstable nuclei together with spin or parity state of excited states of their decayed (daughter) nuclei. These data are known to be useful for experimental investigation into the structure of unstable nuclei far from the stability line. The present study aims to establish a general method applicable to 11 Be and 16 N nuclei. To produce spin polarization, a new method in which the electron spin polarization of Rb is firstly produced by laser pumping, then the electron is transferred to the unstable nuclear beam (RNB) when they passes through the Rb vapor is proposed. Finally the polarized RNB will be implanted into superfluid helium to remain with a long spin-relaxation time. Future experimental set up for the above measurement adopted in the available radioactive nuclear beam facilities is briefly described. (Ohno, S.)

Probing the Magnetic Field Structure in Sgr A* on Black Hole Horizon Scales with Polarized Radiative Transfer Simulations

Energy Technology Data Exchange (ETDEWEB)

Gold, Roman; McKinney, Jonathan C. [Department of Physics and Joint Space-Science Institute, University of Maryland, College Park, MD 20742 (United States); Johnson, Michael D.; Doeleman, Sheperd S. [Harvard-Smithsonian Center for Astrophysics, 60 Garden Street, Cambridge, MA 02138 (United States)

2017-03-10

Magnetic fields are believed to drive accretion and relativistic jets in black hole accretion systems, but the magnetic field structure that controls these phenomena remains uncertain. We perform general relativistic (GR) polarized radiative transfer of time-dependent three-dimensional GR magnetohydrodynamical simulations to model thermal synchrotron emission from the Galactic Center source Sagittarius A* (Sgr A*). We compare our results to new polarimetry measurements by the Event Horizon Telescope (EHT) and show how polarization in the visibility (Fourier) domain distinguishes and constrains accretion flow models with different magnetic field structures. These include models with small-scale fields in disks driven by the magnetorotational instability as well as models with large-scale ordered fields in magnetically arrested disks. We also consider different electron temperature and jet mass-loading prescriptions that control the brightness of the disk, funnel-wall jet, and Blandford–Znajek-driven funnel jet. Our comparisons between the simulations and observations favor models with ordered magnetic fields near the black hole event horizon in Sgr A*, though both disk- and jet-dominated emission can satisfactorily explain most of the current EHT data. We also discuss how the black hole shadow can be filled-in by jet emission or mimicked by the absence of funnel jet emission. We show that stronger model constraints should be possible with upcoming circular polarization and higher frequency (349 GHz) measurements.

Modeling charge polarization voltage for large lithium-ion batteries in electric vehicles

Directory of Open Access Journals (Sweden)

Yan Jiang

2013-06-01

Full Text Available Purpose: Polarization voltage of the lithium-ion battery is an important parameter that has direct influence on battery performance. The paper aims to analyze the impedance characteristics of the lithium-ion battery based on EIS data. Design/methodology/approach: The effects of currents, initial SOC of the battery on charge polarization voltage are investigated, which is approximately linear function of charge current. The change of charge polarization voltage is also analyzed with the gradient analytical method in the SOC domain. The charge polarization model with two RC networks is presented, and parts of model parameters like Ohmic resistance and charge transfer impedance are estimated by both EIS method and battery constant current testing method. Findings: This paper reveals that the Ohmic resistance accounts for much contribution to battery total polarization compared to charge transfer impedance. Practical implications: Experimental results demonstrate the efficacy of the model with the proposed identification method, which provides the foundation for battery charging optimization. Originality/value: The paper analyzed the impedance characteristics of the lithium-ion battery based on EIS data, presented a charge polarization model with two RC networks, and estimated parameters like Ohmic resistance and charge transfer impedance.

Polarization experiments with hadronic and electromagnetic probes

International Nuclear Information System (INIS)

Punjabi, V.

1993-01-01

The following research activities were carried out during the past year Calibration of focal plane polarimeter POMME up to 2.4 GeV at Saturne National Laboratory (LNS) in Saclay. Measurement of tensor analyzing power T 20 and polarization transfer κ 0 at Saturne up to 2.1 GeV in elastic backward dp scattering rvec dp → rvec pd. Measurement of tensor analyzing power T 20 at synchrophasotron in Dubha up to 4.4 Gev in elastic backward dp scattering rvec dp → pd. Resubmission of conditionally Approved G EP proposal 89-14 at CEBAF. Start construction of focal plane polarimeter (FPP) for CEBAF hall A hadron spectrometer. The planned work for the next year includes: Construction of FPP for CEBAF hall A hadron spectrometer; measurement of polarization transfer κ 0 and tensor analyzing power T 20 in elastic backward dp scattering at Saturne; measurements of tensor analyzing power in 1 H( 6 Li,d)X, 1 H( 6 Li,α)X, 1 H( 6 Li,t)X and 1 H( 6 Li, 3 He)X reactions at Saturne; and study of polarization transfer in 2 H(rvec e,e'rvec p)n reaction at Bates

Polarization Measurements in Neutral Pion Photoproduction

International Nuclear Information System (INIS)

C. Jones; Krishni Wijesooriya; B. Fox; Andrei Afanasev; Moscov Amaryan; Konrad Aniol; Stephen Becher; Kamal Benslama; Louis Bimbot; Peter Bosted; Edward Brash; John Calarco; Zhengwei Chai; C. Chang; Ting Chang; Jian-Ping Chen; Seonho Choi; Eugene Chudakov; Steve Churchwell; Domenick Crovelli; Sonja Dieterich; Scott Dumalski; Dipangkar Dutta; Martin Epstein; Kevin Fissum; Salvatore Frullani; Haiyan Gao; Juncai Gao; Franco Garibaldi; Olivier Gayou; Ronald Gilman; Oleksandr Glamazdin; Charles Glashausser; Javier Gomez; Viktor Gorbenko; Ole Hansen; Roy Holt; Jordan Hovdebo; Garth Huber; Kees de Jager; Xiaodong Jiang; Mark Jones; Jim Kelly; Edward Kinney; Edgar Kooijman; Gerfried Kumbartzki; Michael Kuss; John LeRose; Meme Liang; Richard Lindgren; Nilanga Liyanage; Sergey Malov; Demetrius Margaziotis; Pete Markowitz; Kathy McCormick; Dave Meekins; Zein-Eddine Meziani; Robert Michaels; Joe Mitchell; Ludyvine Morand; Charles Perdrisat

2002-01-01

We present measurements of the recoil proton polarization for the 1 H(gamma-vector,p-vector)pi 0 reaction for theta c.m. pi = 60 o -135 o and for photon energies up to 4.1 GeV. These are the first data in this reaction for polarization transfer with circularly polarized photons. Various theoretical models are compared with the results. No evidence for hadron helicity conservation is observed. Models that employ factorization are not favored. It appears from the strong angular dependence of the induced polarization at photon energies of 2.5 and 3.1 GeV that a relatively high spin resonance or background amplitude might exist in this energy region

Simultaneously 'pushing' and 'pulling' graphene oxide into low-polar solvents through a designed interface.

Science.gov (United States)

Liu, Zhen; Liu, Jingquan; Wang, Yichao; Razal, Joselito M; Francis, Paul S; Biggs, Mark J; Barrow, Colin J; Yang, Wenrong

2018-08-03

Dispersing graphene oxide (GO) in low-polar solvents can realize a perfect self-assembly with functional molecules and application in removal of organic impurities that only dissolve in low-polar solvents. The surface chemistry of GO plays an important role in its dispersity in these solvents. The direct transfer of hydrophilic GO into low-polar solvents, however, has remained an experimental challenge. In this study, we design an interface to transfer GO by simultaneously 'pushing and pulling' the nanosheets into low-polar solvents. Our approach is outstanding due to the ability to obtain monolayers of chemically reduced GO (CRGO) with designed surface properties in the organic phase. Using the transferred GO or CRGO dispersions, we have fabricated GO/fullerene nanocomposites and assessed the ability of CRGOs for dye adsorption. We hope our work can provide a universal approach for the phase transfer of other nanomaterials.

Polarization and charge-transfer effect on the transport properties in two-dimensional electron gases/LaNiO3 heterostructure

Science.gov (United States)

Chen, M. J.; Ning, X. K.; Wang, Z. J.; Liu, P.; Wang, S. F.; Wang, J. L.; Fu, G. S.; Ma, S.; Liu, W.; Zhang, Z. D.

2018-01-01

The film thickness dependent transport properties of the LaNiO3 (LNO) layer epitaxially grown on LaAlO3/SrTiO3 (LAO) 2-dimensional electronic gas (2DEG) have been investigated. The ultrathin LNO films grown on the 2DEG have a sheet resistance below the values of h/e2 in all temperature ranges. The electron density is enhanced by more than one order of magnitude by capping LNO films. X-ray photoelectron spectroscopy shows that the interface undergoes unambiguous charge transfer and electronic reconstruction, leading to modulation doping of such atomically engineered complex oxide heterointerfaces. The polar-catastrophe of the 2DEG is directly linked to the electronic structure and transport properties of the LNO. The transport properties can be well modulated by the thickness of the LAO in the 2DEG, and the data can be well fitted with the polar-catastrophe scenario. These results suggest a general approach to tunable functional films in oxide heterostructures with the 2DEG.

Green Wireless Power Transfer Networks

NARCIS (Netherlands)

Liu, Q.; Golinnski, M.; Pawelczak, P.; Warnier, M.

2016-01-01

wireless power transfer network (WPTN) aims to support devices with cable-less energy on-demand. Unfortunately, wireless power transfer itself-especially through radio frequency radiation rectification-is fairly inefficient due to decaying power with distance, antenna polarization, etc.

Markov chain formalism for generalized radiative transfer in a plane-parallel medium, accounting for polarization

Science.gov (United States)

Xu, Feng; Davis, Anthony B.; Diner, David J.

2016-11-01

A Markov chain formalism is developed for computing the transport of polarized radiation according to Generalized Radiative Transfer (GRT) theory, which was developed recently to account for unresolved random fluctuations of scattering particle density and can also be applied to unresolved spectral variability of gaseous absorption as an improvement over the standard correlated-k method. Using Gamma distribution to describe the probability density function of the extinction or absorption coefficient, a shape parameter a that quantifies the variability is introduced, defined as the mean extinction or absorption coefficient squared divided by its variance. It controls the decay rate of a power-law transmission that replaces the usual exponential Beer-Lambert-Bouguer law. Exponential transmission, hence classic RT, is recovered when a→∞. The new approach is verified to high accuracy against numerical benchmark results obtained with a custom Monte Carlo method. For a<∞, angular reciprocity is violated to a degree that increases with the spatial variability, as observed for finite portions of real-world cloudy scenes. While the degree of linear polarization in liquid water cloudbows, supernumerary bows, and glories is affected by spatial heterogeneity, the positions in scattering angle of these features are relatively unchanged. As a result, a single-scattering model based on the assumption of subpixel homogeneity can still be used to derive droplet size distributions from polarimetric measurements of extended stratocumulus clouds.

Linear Polarization, Circular Polarization, and Depolarization of Gamma-ray Bursts: A Simple Case of Jitter Radiation

Energy Technology Data Exchange (ETDEWEB)

Mao, Jirong; Wang, Jiancheng, E-mail: jirongmao@mail.ynao.ac.cn [Yunnan Observatories, Chinese Academy of Sciences, 650011 Kunming, Yunnan Province (China)

2017-04-01

Linear and circular polarizations of gamma-ray bursts (GRBs) have been detected recently. We adopt a simplified model to investigate GRB polarization characteristics in this paper. A compressed two-dimensional turbulent slab containing stochastic magnetic fields is considered, and jitter radiation can produce the linear polarization under this special magnetic field topology. Turbulent Faraday rotation measure (RM) of this slab makes strong wavelength-dependent depolarization. The jitter photons can also scatter with those magnetic clumps inside the turbulent slab, and a nonzero variance of the Stokes parameter V can be generated. Furthermore, the linearly and circularly polarized photons in the optical and radio bands may suffer heavy absorptions from the slab. Thus we consider the polarized jitter radiation transfer processes. Finally, we compare our model results with the optical detections of GRB 091018, GRB 121024A, and GRB 131030A. We suggest simultaneous observations of GRB multi-wavelength polarization in the future.

Three-dimensional Radiative Transfer Simulations of the Scattering Polarization of the Hydrogen Lyalpha Line in a Magnetohydrodynamic Model of the Chromosphere-Corona Transition Region

Czech Academy of Sciences Publication Activity Database

Štěpán, Jiří; Trujillo Bueno, J.; Leenaarts, J.; Carlsson, M.

2015-01-01

Roč. 803, č. 2 (2015), 65/1-65/15 ISSN 0004-637X R&D Projects: GA ČR GPP209/12/P741 Grant - others:EU(XE) COST action MP1104 Institutional support: RVO:67985815 Keywords : polarization * radiative transfer * scattering Subject RIV: BN - Astronomy, Celestial Mechanics, Astrophysics Impact factor: 5.909, year: 2015

Magnetic excitations and polarized neutrons

International Nuclear Information System (INIS)

Shirane, G.

1985-01-01

We review the historical development of polarized beam techniques for studies of condensed matter physics. In particular we describe, in some detail, the recent advance of the triple axis technique with polarization analysis. It is now possible to carry out quantitative characterization of magnetic cross sections S(Q,ω), in absolute units, for a wide range of energy and momentum transfers. We will discuss some examples of recent inelastic measurements on 3d ferromagnets and heavy Fermions. 35 refs., 11 figs., 2 tabs

Spin-locking and cross-polarization under magic-angle spinning of uniformly labeled solids.

Science.gov (United States)

Hung, Ivan; Gan, Zhehong

2015-07-01

Spin-locking and cross-polarization under magic-angle spinning are investigated for uniformly (13)C and (15)N labeled solids. In particular, the interferences from chemical shift anisotropy, and (1)H heteronuclear and (13)C homonuclear dipolar couplings are identified. The physical origin of these interferences provides guidelines for selecting the best (13)C and (15)N polarization transfer rf fields. Optimal settings for both the zero- and double-quantum cross-polarization transfer mechanisms are recommended. Copyright © 2015 Elsevier Inc. All rights reserved.

Polarized radiative transfer through terrestrial atmosphere accounting for rotational Raman scattering

Science.gov (United States)

Lelli, Luca; Rozanov, Vladimir V.; Vountas, Marco; Burrows, John P.

2017-10-01

This paper is devoted to the phenomenological derivation of the vector radiative transfer equation (VRTE) accounting for first-order source terms of rotational Raman scattering (RRS), which is responsible for the in-filling of Fraunhofer and telluric lines by inelastic scattered photons. The implementation of the solution of the VRTE within the framework of the forward-adjoint method is given. For the Ca II and the oxygen A-band (O2 A) spectral windows, values of reflectance, degree of linear polarization (DOLP) and in-filling, in zenith and nadir geometry, are compared with results given in literature. Moreover, the dependence of these quantities on the columnar loading and vertical layering of non-spherical dust aerosols is investigated, together with their changes as function of two habits of ice crystals, modeled as regular icosahedra and severely rough aggregated columns. Bi-directional effects of an underlying polarizing surface are accounted for. The forward simulations are performed for one selected wavelength in the continuum and one in the strong absorption of the O2 A, as their combination can be exploited for the spaceborne retrieval of aerosol and cloud properties. For this reason, we also mimic seasonal maps of reflectance, DOLP and in-filling, that are prototypical measurements of the Ultraviolet-Visible-Near Infrared (UVN) sensor, at a nominal spectral resolution of 0.12 nm. UVN is the core payload of the upcoming European Sentinel-4 mission, that will observe Europe in geostationary orbit for air quality monitoring purposes. In general, in the core of O2 A, depending on the optical thickness and altitude of the scatterers, we find RRS-induced in-filling values ranging from 1.3% to 1.8%, while DOLP decreases by 1%. Conversely, while negligible differences of RRS in-filling are calculated with different ice crystal habits, the severely rough aggregated column model can reduce DOLP by a factor up to 10%. The UVN maps of in-filling show values varying

Dynamic Nuclear Polarization and other magnetic ideas at EPFL.

Science.gov (United States)

Bornet, Aurélien; Milani, Jonas; Wang, Shutao; Mammoli, Daniele; Buratto, Roberto; Salvi, Nicola; Segaw, Takuya F; Vitzthum, Veronika; Miéville, Pascal; Chinthalapalli, Srinivas; Perez-Linde, Angel J; Carnevale, Diego; Jannin, Sami; Caporinia, Marc; Ulzega, Simone; Rey, Martial; Bodenhausen, Geoffrey

2012-01-01

Although nuclear magnetic resonance (NMR) can provide a wealth of information, it often suffers from a lack of sensitivity. Dynamic Nuclear Polarization (DNP) provides a way to increase the polarization and hence the signal intensities in NMR spectra by transferring the favourable electron spin polarization of paramagnetic centres to the surrounding nuclear spins through appropriate microwave irradiation. In our group at EPFL, two complementary DNP techniques are under investigation: the combination of DNP with magic angle spinning at temperatures near 100 K ('MAS-DNP'), and the combination of DNP at 1.2 K with rapid heating followed by the transfer of the sample to a high-resolution magnet ('dissolution DNP'). Recent applications of MAS-DNP to surfaces, as well as new developments of magnetization transfer of (1)H to (13)C at 1.2 K prior to dissolution will illustrate the work performed in our group. A second part of the paper will give an overview of some 'non-enhanced' activities of our laboratory in liquid- and solid-state NMR.

Elimination of polarity in the carotenoid terminus promotes the exposure of B850-binding sites (Tyr 44, 45) and ANS-mediated energy transfer in LH2 complexes of Rhodobacter sphaeroides.

Science.gov (United States)

Liu, Yuan; Wu, Yongqiang; Xu, Chunhe

2004-12-10

Carotenoids in the peripheral light-harvesting complexes (LH2) of the green mutant (GM309) of Rhodobacter sphaeroides were identified as containing neurosporenes, which lack the polar CH(3)O group, compared to spheroidenes in native-LH2 of R. sphaeroides 601. After LH2 complexes were treated with 1-anilino-8-naphthalene sulfonate (ANS), new energy transfer pathways from ANS or tryptophan to carotenoids were discovered in both native- and GM309-LH2. The carotenoid fluorescence intensity of GM309-LH2 was greater than that of native-LH2 when bound with ANS, suggesting that the elimination of polarity in the neurosporene increases the energy transfer from ANS to carotenoid. The fact that two alpha-tyrosines (alpha-Tyr 44, 45, B850-binding sites) in each alpha-apoprotein of GM309-LH2 were more easily modified than those of native-LH2 by N-acetylimidazole (NAI) indicates that the elimination of polarity in the neurosporene terminus increases the exposure of these sites to solution.

POLARIZED LINE FORMATION IN NON-MONOTONIC VELOCITY FIELDS

Energy Technology Data Exchange (ETDEWEB)

Sampoorna, M.; Nagendra, K. N., E-mail: sampoorna@iiap.res.in, E-mail: knn@iiap.res.in [Indian Institute of Astrophysics, Koramangala, Bengaluru 560034 (India)

2016-12-10

For a correct interpretation of the observed spectro-polarimetric data from astrophysical objects such as the Sun, it is necessary to solve the polarized line transfer problems taking into account a realistic temperature structure, the dynamical state of the atmosphere, a realistic scattering mechanism (namely, the partial frequency redistribution—PRD), and the magnetic fields. In a recent paper, we studied the effects of monotonic vertical velocity fields on linearly polarized line profiles formed in isothermal atmospheres with and without magnetic fields. However, in general the velocity fields that prevail in dynamical atmospheres of astrophysical objects are non-monotonic. Stellar atmospheres with shocks, multi-component supernova atmospheres, and various kinds of wave motions in solar and stellar atmospheres are examples of non-monotonic velocity fields. Here we present studies on the effect of non-relativistic non-monotonic vertical velocity fields on the linearly polarized line profiles formed in semi-empirical atmospheres. We consider a two-level atom model and PRD scattering mechanism. We solve the polarized transfer equation in the comoving frame (CMF) of the fluid using a polarized accelerated lambda iteration method that has been appropriately modified for the problem at hand. We present numerical tests to validate the CMF method and also discuss the accuracy and numerical instabilities associated with it.

Time Domain Induced Polarization

DEFF Research Database (Denmark)

Fiandaca, Gianluca; Auken, Esben; Christiansen, Anders Vest

2012-01-01

Time-domain-induced polarization has significantly broadened its field of reference during the last decade, from mineral exploration to environmental geophysics, e.g., for clay and peat identification and landfill characterization. Though, insufficient modeling tools have hitherto limited the use...... of time-domaininduced polarization for wider purposes. For these reasons, a new forward code and inversion algorithm have been developed using the full-time decay of the induced polarization response, together with an accurate description of the transmitter waveform and of the receiver transfer function......, to reconstruct the distribution of the Cole-Cole parameters of the earth. The accurate modeling of the transmitter waveform had a strong influence on the forward response, and we showed that the difference between a solution using a step response and a solution using the accurate modeling often is above 100...

Studies of nuclear structure via polarization transfer experiments

International Nuclear Information System (INIS)

Moss, J.M.

1985-01-01

Inelastic scattering and charge exchange reactions at medium energies are discussed. Theoretical treatments of these phenomena based on the Dirac equation are presented. A LAMPF experiment in which polarization observables were employed in the search for collective effects in the nuclear pion field is discussed. This experiment is compared with the EMC (European Muon Collaboration) effect. 37 refs., 11 figs

A FORMALISM FOR COVARIANT POLARIZED RADIATIVE TRANSPORT BY RAY TRACING

International Nuclear Information System (INIS)

Gammie, Charles F.; Leung, Po Kin

2012-01-01

We write down a covariant formalism for polarized radiative transfer appropriate for ray tracing through a turbulent plasma. The polarized radiation field is represented by the polarization tensor (coherency matrix) N αβ ≡ (a α k a* β k ), where a k is a Fourier coefficient for the vector potential. Using Maxwell's equations, the Liouville-Vlasov equation, and the WKB approximation, we show that the transport equation in vacuo is k μ ∇ μ N αβ = 0. We show that this is equivalent to Broderick and Blandford's formalism based on invariant Stokes parameters and a rotation coefficient, and suggest a modification that may reduce truncation error in some situations. Finally, we write down several alternative approaches to integrating the transfer equation.

APC: A New Code for Atmospheric Polarization Computations

Science.gov (United States)

Korkin, Sergey V.; Lyapustin, Alexei I.; Rozanov, Vladimir V.

2014-01-01

A new polarized radiative transfer code Atmospheric Polarization Computations (APC) is described. The code is based on separation of the diffuse light field into anisotropic and smooth (regular) parts. The anisotropic part is computed analytically. The smooth regular part is computed numerically using the discrete ordinates method. Vertical stratification of the atmosphere, common types of bidirectional surface reflection and scattering by spherical particles or spheroids are included. A particular consideration is given to computation of the bidirectional polarization distribution function (BPDF) of the waved ocean surface.

Measurement of polarization observables of the associated strangeness production in proton proton interactions

Energy Technology Data Exchange (ETDEWEB)

Hauenstein, F.; Klaja, P. [Forschungszentrum Juelich, Institut fuer Kernphysik, Juelich (Germany); Friedrich-Alexander-Universitaet Erlangen-Nuernberg, Erlangen (Germany); Borodina, E.; Dzhygadlo, R.; Gast, W.; Gillitzer, A.; Grzonka, D.; Kilian, K.; Mertens, M.; Roderburg, E.; Roeder, M.; Sefzick, T.; Wintz, P. [Forschungszentrum Juelich, Institut fuer Kernphysik, Juelich (Germany); Clement, H.; Doroshkevich, E.; Ehrhardt, K. [Physikalisches Institut der Universitaet Tuebingen, Tuebingen (Germany); University of Tuebingen, Kepler Center for Astro and Particle Physics, Tuebingen (Germany); Eyrich, W.; Kober, L.; Krapp, M. [Friedrich-Alexander-Universitaet Erlangen-Nuernberg, Erlangen (Germany); Jowzaee, S. [Forschungszentrum Juelich, Institut fuer Kernphysik, Juelich (Germany); Jagellonian University, Institute of Physics, Cracow (Poland); Moskal, P.; Smyrski, J. [Jagellonian University, Institute of Physics, Cracow (Poland); Ritman, J. [Forschungszentrum Juelich, Institut fuer Kernphysik, Juelich (Germany); Juelich Aachen Research Alliance, Forces and Matter Experiments (JARA-FAME), Forschungszentrum Juelich, Juelich (Germany); RWTH Aachen, Aachen (Germany); Ruhr-Universitaet Bochum, Experimentalphysik I, Bochum (Germany); Schroeder, W. [Forschungszentrum Juelich, Corporate Development, Juelich (Germany); Wuestner, P. [Zentralinstitut fuer Engineering, Elektronik und Analytik, Juelich (Germany); Collaboration: The COSY-TOF Collaboration

2016-11-15

The Λ polarization, the analyzing power, and the Λ spin transfer coefficient of the reaction pp → pK{sup +} Λ were measured at beam momenta of 2.70 GeV/c and 2.95 GeV/c corresponding to excess energies of 122 MeV and 204 MeV. While the analyzing power and the spin transfer coefficient do not change significantly with the excess energy, the Λ polarization varies strongly and changes its sign. As this is the first measurement of polarization observables below an excess energy of 200 MeV, the change of the sign of the Λ polarization was not observed before. The high statistics of the data (∼ 200 k events for each momentum) enables detailed studies of the dependence of the Λ polarization and the analyzing power on the center-of-mass momentum of the particles. The results of the spin transfer coefficient are in qualitative agreement with the DISTO experiment. The Λ polarization data of 2.95 GeV/c are only conform with the DISTO experiment, while both the 2.70 GeV/c and 2.95 GeV/c data differ strongly from all previous measurements, whether exclusive or inclusive. (orig.)

The Polar Cusp

International Nuclear Information System (INIS)

Holtet, J.A.; Egeland, A.

1985-01-01

The upper atmosphere at high latitudes is often called the ''earth's window to outer space.'' Through various electrodynamic coupling processes, as well as direct transfer of particles, many of the geophysical effects displayed are direct manifestations of phenomena occurring in deep space. The high latitude ionosphere also exerts a feedback on the regions of the magnetosphere and atmosphere to which it is coupled. Of particular interest are the sections of the near space known as the Polar Cusp. A vast portion of the Earth's magnetic field envelope is electrically connected to these regions. This geometry results in a spatial mapping of the magnetospheric processes and a focusing on the ionosphere. In the Polar Cusps, the solar wind plasma also has direct access to the upper atmosphere

A high volume, batch mode {sup 129}Xe polarizer

Energy Technology Data Exchange (ETDEWEB)

Wojna-Pelczar, Anna, E-mail: anna.wojna.pelczar@mail.muni.cz [Central European Institute of Technology, Masaryk University, Brno (Czech Republic); Formerly: Marian Smoluchowski Institute of Physics, Jagiellonian University, Kraków (Poland); Pałasz, Tadeusz [Marian Smoluchowski Institute of Physics, Jagiellonian University, Kraków (Poland)

2017-06-01

Numerous designs of optical gas polarizers have been proposed, broadening possible applications of the hyperpolarized gases as contrast agents in magnetic resonance imaging. We present a home–made {sup 129}Xe polarizer based on the spin exchange optical pumping method. The polarizer operates under 1 bar of the gas mixture (at the maximum temperature of 160 °C) in a high volume optical cell (5025 cm{sup 3}). Approximately 100 cm{sup 3} of {sup 129}Xe polarized at 1.50±0.37% is produced in a single cycle of polarization. Operation under standard pressure imposes polarization transfer mainly via van der Waals molecules, resulting in the efficient spin exchange between rubidium and {sup 129}Xe atoms. The design, construction and operation of the polarizer are described in details.

Ground-based Polarization Remote Sensing of Atmospheric Aerosols and the Correlation between Polarization Degree and PM2.5

International Nuclear Information System (INIS)

Cheng, Chen; Zhengqiang, Li; Weizhen, Hou; Yisong, Xie; Donghui, Li; Kaitao, Li; Ying, Zhang

2014-01-01

The ground-based polarization remote sensing adds the polarization dimension information to traditional intensity detection, which provides a new method to detect atmospheric aerosols properties. In this paper, the polarization measurements achieved by a new multi-wavelength sun photometer, CE318-DP, are used for the ground-based remote sensing of atmospheric aerosols. In addition, a polarized vector radiative transfer model is introduced to simulate the DOLP (Degree Of Linear Polarization) under different sky conditions. At last, the correlative analysis between mass density of PM 2.5 and multi-wavelength and multi-angular DOLP is carried out. The result shows that DOLP has a high correlation with mass density of PM 2.5 , R 2 >0.85. As a consequence, this work provides a new method to estimate the mass density of PM 2.5 by using the comprehensive network of ground-based sun photometer

[The Effect of Observation Geometry on Polarized Skylight Spectrum].

Science.gov (United States)

Zhang, Ren-bin; Wang, Ling-mei; Gao, Jun; Wang, Chi

2015-03-01

Study on polarized skylight spectral characters while observation geometry changing in different solar zenith angles (SZA), viewing zenith angles (VZA) or relative azimuth angles (RAA). Simulation calculation of cloudless daylight polarimetric spectrum is realized based on the solver, vector discrete ordinate method, of radiative transfer equation. In the Sun's principal and perpendicular plane, the spectral irradiance data, varying at wavelengths in the range between 0.4 and 3 μm, are calculated to extend the atmospheric polarization spectral information under the conditions: the MODTRAN solar reference spectrur is the only illuminant source; the main influencing factors of polarized radiative transfer include underlying surface albedo, aerosol layers and components, and the absorption of trace gases. Simulation analysis results: (1) While the relative azimuth angle is zero, the magnitude of spectrum U/I is lower than 10(-7) and V/I is negligible, the degree of polarization and the spectrum Q/I are shaped like the letter V or mirror-writing U. (2) In twilight, when the Sun is not in FOV of the detector, the polarization of the daytime sky has two maximum near 0.51 and 2.75 μm, and a minimum near 1.5 μm. For arbitrary observation geometry, the spectral signal of V/I may be ignored. According to observation geometry, choosing different spectral bands or polarized signal will be propitious to targets detection.

Competitive photocyclization/rearrangement of 4-aryl-1,1-dicyanobutenes controlled by intramolecular charge-transfer interaction. Effect of medium polarity, temperature, pressure, excitation wavelength, and confinement.

Science.gov (United States)

Ito, Tadashi; Nishiuchi, Emi; Fukuhara, Gaku; Inoue, Yoshihisa; Mori, Tadashi

2011-09-01

A series of 4-aryl-1,1-dicyanobutenes (1a-1f) with different substituents were synthesized to control the intramolecular donor-acceptor or charge-transfer (C-T) interactions in the ground state. Photoexcitation of these C-T substrates led to competitive cyclization and rearrangement, the ratio being critically controlled by various environmental factors, such as solvent polarity, temperature and static pressure, and also by excitation wavelength and supramolecular confinement (polyethylene voids). In non-polar solvents, the rearrangement was dominant (>10 : 1) for all examined substrates, while the cyclization was favoured in polar solvents, in particular at low temperatures. Selective excitation at the C-T band further enhanced the cyclization up to >50 : 1 ratios. More importantly, the cyclization/rearrangement ratio was revealed to be a linear function of the C-T transition energy. However, the substrates with a sterically demanding or highly electron-donating substituent failed to give the cyclization product.

Radially Polarized Conical Beam from an Embedded Etched Fiber

OpenAIRE

Kalaidji , D.; Spajer , M.; Marthouret , N.; Grosjean , T.

2009-01-01

International audience; We propose a method for producing a conical beam based on the lateral refraction of the TM01 mode from a two-mode fiber after chemical etching of the cladding, and for controlling its radial polarization. The whole power of the guided mode is transferred to the refracted beam with low diffraction. Polarization control by a series of azimuthal detectors and a stress controller affords the transmission of a stabilized radial polarization through an optical fiber. A solid...

Dynamical nuclear polarization using multi-colour control of color centers in diamond

Energy Technology Data Exchange (ETDEWEB)

Yang, Pengcheng [Huazhong University of Science and Technology, School of Physics, Wuhan (China); Huazhong University of Science and Technology, Center for Quantum Optical Science, Wuhan (China); Plenio, Martin B. [Universitaet Ulm, Institut fuer Theoretische Physik, Ulm (Germany); Universitaet Ulm, Center for Integrated Quantum Science and Technology, Ulm (Germany); Cai, Jianming [Huazhong University of Science and Technology, School of Physics, Wuhan (China); Huazhong University of Science and Technology, Center for Quantum Optical Science, Wuhan (China); Universitaet Ulm, Institut fuer Theoretische Physik, Ulm (Germany); Universitaet Ulm, Center for Integrated Quantum Science and Technology, Ulm (Germany)

2016-12-15

Dynamical nuclear polarization (DNP) transfers the polarization of electron spins at cryogenic temperatures to achieve strong nuclear polarization for applications in nuclear magnetic resonance. Recently introduced approaches employ optical pumping of nitrogen-vacancy (NV) centers in diamond to achieve DNP even at ambient temperatures. In such schemes microwave radiation is used to establish a Hartmann-Hahn condition between the NV electron spin and proximal nuclear spins to facilitate polarization transfer. For a single monochromatic microwave driving field, the Hartmann-Hahn condition cannot be satisfied for an ensemble of NV centers due to inhomogeneous broadening and reduces significantly the overall efficiency of dynamical nuclear polarization using an ensemble of NV centers. Here, we adopt generalized Hartmann-Hahn type dynamical nuclear polarization schemes by applying microwave driving fields with (multiple) time-modulated frequencies. We show that it is possible to enhance the effective coupling between an ensemble of NV center spins with inhomogeneous broadening and nuclear spins, thereby improving significantly the overall efficiency of dynamical nuclear polarization. This approach can also be used to achieve dynamical nuclear polarization of an ensemble of nuclei with a distribution of Larmor frequencies, which would be helpful in magnetic resonance spectroscopy using a single NV spin sensor. (orig.)

High-efficiency transmision neutron polarizer for high-resolution double crystal diffractometer

International Nuclear Information System (INIS)

Ioffe, A.; Krist, T.; Mezei, F.; Gordeev, G.; Ibrayev, B.

1997-01-01

An efficient transmission geometry neutron polarizer for the high-resolution double crystal diffractometer at HMI (λ=4.8 A) is described. A polarization of about 94% was achieved and the polarized neutron beam intensity amounts to 40% of the nonpolarized beam intensity. This opens up wide possibilities for the study of magnetic small-angle scattering for extremely small momentum transfer (Q∝10 -5 A -1 ). (orig.)

Interfacial polarization phenomena in organic molecular films

International Nuclear Information System (INIS)

Iwamoto, Mitsumasa; Manaka, Takaaki

2006-01-01

Electrostatic phenomena occurring at the interface between metal/organic and organic/organic materials are discussed from the viewpoint of dielectrics physics. Focusing on two important origins of surface polarization phenomena, orientational ordering of polar molecules and displacement of excess charges at the interface, surface polarization phenomena of organic thin films are discussed. To define the orientational order of polar molecules, orientational order parameters are introduced, and surface polarization due to the alignment of dipoles is expressed. The generation of Maxwell displacement current (MDC) and optical second harmonic generation (SHG) that are specific for surface organic monomolecular films are discussed, and some experimental evidence are shown. As an extension of the concept of surface Fermi level introduced to discuss the electrostatic phenomena due to electron transfer at the interface between metal-organic insulators, the surface Fermi level is extended to the discussion on the electrostatic phenomena of organic semiconductor materials on metals. In this paper, some experimental evidence of surface polarization originating from polar molecules and displacement of excess charges are shown. After that, with consideration of these surface phenomena, single electron tunneling of organic films are briefly discussed in association with surface polarization phenomena

Effect of anode polarization on biofilm formation and electron transfer in Shewanella oneidensis/graphite felt microbial fuel cells.

Science.gov (United States)

Pinto, David; Coradin, Thibaud; Laberty-Robert, Christel

2018-04-01

In microbial fuel cells, electricity generation is assumed by bacterial degradation of low-grade organics generating electrons that are transferred to an electrode. The nature and efficiency of the electron transfer from the bacteria to the electrodes are determined by several chemical, physical and biological parameters. Specifically, the application of a specific potential at the bioanode has been shown to stimulate the formation of an electro-active biofilm, but the underlying mechanisms remain poorly understood. In this study, we have investigated the effect of an applied potential on the formation and electroactivity of biofilms established by Shewanella oneidensis bacteria on graphite felt electrodes in single- and double-chamber reactor configurations in oxic conditions. Using amperometry, cyclic voltammetry, and OCP/Power/Polarization curves techniques, we showed that a potential ranging between -0.3V and +0.5V (vs. Ag/AgCl/KCl sat.) and its converse application to a couple of electrodes leads to different electrochemical behaviors, anodic currents and biofilm architectures. For example, when the bacteria were confined in the anodic compartment of a double-chamber cell, a negative applied potential (-0.3V) at the bioanode favors a mediated electron transfer correlated with the progressive formation of a biofilm that fills the felt porosity and bridges the graphite fibers. In contrast, a positive applied potential (+0.3V) at the bioanode stimulates a direct electron transfer resulting in the fast-bacterial colonization of the fibers only. These results provide significant insight for the understanding of the complex bacteria-electrode interactions in microbial fuel cells. Copyright © 2017 Elsevier B.V. All rights reserved.

Spin-isospin excitations studied by polarized beams

International Nuclear Information System (INIS)

Sakai, H.; Greenfield, M.B.; Hatanaka, K.

1996-01-01

The spin-parity J π of the spin dipole resonances (SDR) in 12 N and 12 B are investigated via the measurements of polarization observables, the transverse polarization transfer coefficient D NN for the (vector p, vector n) reaction at 197 and 295 MeV and the tensor analyzing power A xx for the (vector d, 2 He) reaction at 270 MeV. The polarization observables, D NN and A xx for the peak at 4.5 MeV are consistent with the DWIA prediction with 2 - but those for the peak at 7.5 MeV contradict the predictions with an expected J π =1 - . Neither polarization observables could detect any concentration of 0 - strength. The usefulness of these spin observables in identifying J π is shown. (orig.)

Spin polarized electron source technology transferred from HE accelerators to electron microscopes

International Nuclear Information System (INIS)

Nakanishi, Tsutomu

2009-01-01

For many years, we have developed a technology of spin-polarized-electron-source (PES) for a future linear collider project (ILC). Various new techniques for achieving high polarization, high quantum efficiency, high current density, sub-nanosecond multi-bunch generation etc. were developed. Two fundamental technologies; reduction of dark current and preparation of extremely high vacuum environment to protect the Negative Electron Affinity (NEA) surface have been also developed. Using these PES technologies and a new transmission type photocathode, we recently succeeded in producing the high brightness and high polarization electron beam for the low energy electron microscope (LEEM). Our Spin-LEEM system enables the world-first dynamic observation of surface magnetic domain formed by evaporation on the metal substrate with ∼ 20 nm space resolutions. (author)

Radially polarized conical beam from an embedded etched fiber.

Science.gov (United States)

Kalaidji, Djamel; Spajer, Michel; Marthouret, Nadège; Grosjean, Thierry

2009-06-15

We propose a method for producing a conical beam based on the lateral refraction of the TM(01) mode from a two-mode fiber after chemical etching of the cladding, and for controlling its radial polarization. The whole power of the guided mode is transferred to the refracted beam with low diffraction. Polarization control by a series of azimuthal detectors and a stress controller affords the transmission of a stabilized radial polarization through an optical fiber. A solid component usable for many applications has been obtained.

Deterministic and stochastic methods of calculation of polarization characteristics of radiation in natural environment

Science.gov (United States)

Strelkov, S. A.; Sushkevich, T. A.; Maksakova, S. V.

2017-11-01

We are talking about russian achievements of the world level in the theory of radiation transfer, taking into account its polarization in natural media and the current scientific potential developing in Russia, which adequately provides the methodological basis for theoretically-calculated research of radiation processes and radiation fields in natural media using supercomputers and mass parallelism. A new version of the matrix transfer operator is proposed for solving problems of polarized radiation transfer in heterogeneous media by the method of influence functions, when deterministic and stochastic methods can be combined.

Polarized ionic source of the tandem accelerator in Kyoto University

Energy Technology Data Exchange (ETDEWEB)

Nakamura, Masanobu; Kuwamoto, Shuichi; Takahashi, Seiji [Kyoto Univ. (Japan). Dept. of Physics] [and others

1997-02-01

A polarized ion source developed under the National Laboratory of High Energy Physics was transferred to the tandem accelerator in Kyoto University at beginning of 1993 to constitute a displacement of incidence into the accelerator. This was an atomic beam type polarized ion source, which is designed to adopt permanent magnets for 6 poles magnet to polarize the electron, to take out atomic nucleus on a shape of positive ion by ECR ionizer after transferring its polarization through transition using radio frequency (RFT), to make it negative ion by charge conversion using alkaline metal vapor, and to put it into the tandem accelerator. Test of the positive ion was finished at the National Laboratory of High Energy Physics, and test in Kyoto University was required after its negative ionization. As the estimated cost was unsufficient and entrance into the ion source facility in the tandem accelerator building was limited in Kyoto University, step of development was slow. Here is reported on present state of the ion source which is now operating stably. (G.K.)

Polarization versus Temperature in Pyridinium Ionic Liquids

DEFF Research Database (Denmark)

Chaban, V. V.; Prezhdo, O. V.

2014-01-01

Electronic polarization and charge transfer effects play a crucial role in thermodynamic, structural, and transport properties of room-temperature ionic liquids (RTILs). These nonadditive interactions constitute a useful tool for tuning physical chemical behavior of RTILs. Polarization and charge...... interactions changes negligibly between 300 and 900 K, while the average dipole moment increases due to thermal fluctuations of geometries. Our results contribute to the fundamental understanding of electronic effects in the condensed phase of ionic systems and foster progress in physical chemistry...

Voltammetry of ion transfer across a polarized room-temperature ionic liquid membrane facilitated by valinomycin: theoretical aspects and application.

Science.gov (United States)

Langmaier, Jan; Samec, Zdenek

2009-08-01

Cyclic voltammetry is used to investigate the transfer of alkali-metal cations, protons, and ammonium ions facilitated by the complex formation with valinomycin at the interface between an aqueous electrolyte solution and a room-temperature ionic liquid (RTIL) membrane. The membrane is made of a thin (approximately 112 microm) microporous filter impregnated with an RTIL that is composed of tridodecylmethylammonium cations and tetrakis[3,5-bis(trifluoromethyl)phenyl]borate anions. An extension of the existing theory of voltammetry of ion transfer across polarized liquid membranes makes it possible to evaluate the standard ion-transfer potentials for the hydrophilic cations studied, as well as the stability constants (K(i)) of their 1:1 complexes with valinomycin, as log K(i) = 9.0 (H(+)), 11.1 (Li(+)), 12.8 (Na(+)), 17.2 (K(+)), 15.7 (Rb(+)), 15.1 (Cs(+)), and 14.7 (NH(4)(+)). These data point to the remarkably enhanced stability of the valinomycin complexes within RTIL, and to the enhanced selectivity of valinomycin for K(+) over all other univalent ions studied, compared to the conventional K(+) ion-selective liquid-membrane electrodes. Selective complex formation allows one to resolve voltammetric responses of K(+) and Na(+) in the presence of an excess of Mg(2+) or Ca(2+), which is demonstrated by determination of K(+) and Na(+) in the table and tap water samples.

Vacuum polarization and renormalized charge in ν-dimensions

International Nuclear Information System (INIS)

Marinho Junior, R.M.; Lucinda, J.

1984-01-01

The expression for the vacuum polarization is obtained for any momentum transfer in ν dimensions. Using the Wilson loop for QED, the renormalized electric charge in ν dimensions is calculated. (Author) [pt

Calibration of the degree of linear polarization measurements of the polarized Sun-sky radiometer based on the POLBOX system.

Science.gov (United States)

Li, Zhengqiang; Li, Kaitao; Li, Li; Xu, Hua; Xie, Yisong; Ma, Yan; Li, Donghui; Goloub, Philippe; Yuan, Yinlin; Zheng, Xiaobing

2018-02-10

Polarization observation of sky radiation is the frontier approach to improve the remote sensing of atmospheric components, e.g., aerosol and clouds. The polarization calibration of the ground-based Sun-sky radiometer is the basis for obtaining accurate degree of linear polarization (DOLP) measurement. In this paper, a DOLP calibration method based on a laboratory polarized light source (POLBOX) is introduced in detail. Combined with the CE318-DP Sun-sky polarized radiometer, a calibration scheme for DOLP measurement is established for the spectral range of 440-1640 nm. Based on the calibration results of the Sun-sky radiometer observation network, the polarization calibration coefficient and the DOLP calibration residual are analyzed statistically. The results show that the DOLP residual of the calibration scheme is about 0.0012, and thus it can be estimated that the final DOLP calibration accuracy of this method is about 0.005. Finally, it is verified that the accuracy of the calibration results is in accordance with the expected results by comparing the simulated DOLP with the vector radiative transfer calculations.

A method to calculate Stokes parameters and angle of polarization of skylight from polarized CIMEL sun/sky radiometers

International Nuclear Information System (INIS)

Li, L.; Li, Z.; Li, K.; Blarel, L.; Wendisch, M.

2014-01-01

The polarized CIMEL sun/sky radiometers have been routinely operated within the Sun/sky-radiometer Observation NETwork (SONET) in China and some sites of the AErosol RObotic NETwork (AERONET) around the world. However, the polarization measurements are not yet widely used due to in a certain degree the lack of Stokes parameters derived directly from these polarization measurements. Meanwhile, it have been shown that retrievals of several microphysical properties of aerosol particles can be significantly improved by using degree of linear polarization (DoLP) measurements of polarized CIMEL sun/sky radiometers (CE318-DP). The Stokes parameters Q and U, as well as angle of polarization (AoP) contain additional information about linear polarization and its orientation. A method to calculate Stokes parameters Q, U, and AoP from CE318-DP polarized skylight measurements is introduced in this study. A new polarized almucantar geometry based on CE318-DP is measured to illustrate abundant variation features of these parameters. The polarization parameters calculated in this study are consistent with previous results of DoLP and I, and also comparable to vector radiative transfer simulations. - Highlights: • The CE318-DP polarized measurements are not yet widely used except DoLP. • Compared with DoLP and I, difficulty in calculating Stokes Q and U is discussed. • A new polarized almucantar observation geometry based on CE318-DP is executed. • We derive Stokes Q, U, and AoP both in principal and almucantar plane geometries. • The results are comparable with previous DoLP and I, as well as model simulations

Asymptotic theory of circular polarization memory.

Science.gov (United States)

Dark, Julia P; Kim, Arnold D

2017-09-01

We establish a quantitative theory of circular polarization memory, which is the unexpected persistence of the incident circular polarization state in a strongly scattering medium. Using an asymptotic analysis of the three-dimensional vector radiative transfer equation (VRTE) in the limit of strong scattering, we find that circular polarization memory must occur in a boundary layer near the portion of the boundary on which polarized light is incident. The boundary layer solution satisfies a one-dimensional conservative scattering VRTE. Through a spectral analysis of this boundary layer problem, we introduce the dominant mode, which is the slowest-decaying mode in the boundary layer. To observe circular polarization memory for a particular set of optical parameters, we find that this dominant mode must pass three tests: (1) this dominant mode is given by the largest, discrete eigenvalue of a reduced problem that corresponds to Fourier mode k=0 in the azimuthal angle, and depends only on Stokes parameters U and V; (2) the polarization state of this dominant mode is largely circular polarized so that |V|≫|U|; and (3) the circular polarization of this dominant mode is maintained for all directions so that V is sign-definite. By applying these three tests to numerical calculations for monodisperse distributions of Mie scatterers, we determine the values of the size and relative refractive index when circular polarization memory occurs. In addition, we identify a reduced, scalar-like problem that provides an accurate approximation for the dominant mode when circular polarization memory occurs.

A 1.5--4 Kelvin detachable cold-sample transfer system: Application to inertially confined fusion with spin-polarized hydrogens fuels

International Nuclear Information System (INIS)

Alexander, N.; Barden, J.; Fan, Q.; Honig, A.

1990-01-01

A compact cold-transfer apparatus for engaging and retrieving samples at liquid helium temperatures (1.5--4K), maintaining the samples at such temperatures for periods of hours, and subsequently inserting them in diverse apparatuses followed by disengagement, is described. The properties of several thermal radiation-insulating shrouds, necessary for very low sample temperatures, are presented. The immediate intended application is transportable target-shells containing highly spin-polarized deuterons in solid HD or D 2 for inertially confined fusion (ICF) experiments. The system is also valuable for unpolarized high-density fusion fuels, as well as for other applications which are discussed. 9 refs., 6 figs

Fusion with highly spin polarized HD and D2

International Nuclear Information System (INIS)

Honig, A.; Letzring, S.; Skupsky, S.

1993-01-01

The experimental efforts over the past 5 years have been aimed at carrying out ICF shots with spin-polarized D fuel. The authors successfully prepared polarized D in HD, and solved the problems of loading target shells with their carefully prepared isotopic mixtures, polarizing them so that the D polarization remains metastably frozen-in for about half a day, and carrying out the various cold transfer requirements at Syracuse, where the target is prepared, and at Rochester, where the cold target is inserted into the OMEGA fusion chamber. A principal concern during this past year was overcoming difficulties encountered in maintaining the integrity of the fragile cold target during the multitude of cold-transfers required for the experiment. These difficulties arose from insufficient rigidity of the cold transfer systems, which were constrained to be of small diameter by the narrow central access bore of the dilution refrigerator, and were exacerbated by the multitude of required target shell manipulations between different environments, each with different coupling geometry, including target shell permeation, polarization, storage, transport, retrieval and insertion into OMEGA. The authors did solve all of these problems, and were able to position a cold, high density but unpolarized target with required precision in OMEGA. Upon shooting the accurately positioned unpolarized high density cold target, no neutron yield was observed. Inspection inside the OMEGA tank after the shot indicated the absence of neutron yield was due to mal-timing or insufficient retraction rate of OMEGA's fast shroud mechanism, resulting in interception of at least 20 of the 24 laser beams by the faulty shroud. In spite of this, all elements of the complex experiment the authors originally undertook have been successfully demonstrated, and the cold retrieval concepts and methods they developed are being utilized on the ICF upgrades at Rochester and at Livermore

Variety of Polarized Line Profiles in Interacting Supernovae

Science.gov (United States)

Hoffman, Jennifer L.; Huk, L. N.; Peters, C. L.

2013-01-01

The dense circumstellar material that creates strong emission lines in the spectra of interacting supernovae also gives rise to complex line polarization behavior. Viewed in polarized light, the emission line profiles of these supernovae encode information about the geometrical and optical characteristics of their surrounding circumstellar material (CSM) that is inaccessible by other observational techniques. To facilitate quantitative interpretation of these spectropolarimetric signatures, we have created a large grid of model polarized line profiles using a three-dimensional radiative transfer code that simulates polarization via electron and resonant/fluorescent line scattering. The simulated polarized lines take on an array of profile shapes that vary with viewing angle and CSM properties. We present the major results from the grid and investigate the dependence of polarized line profiles on CSM characteristics including temperature, optical depth, and geometry. These results will allow more straightforward interpretation of polarized line profiles in interacting supernovae than has previously been possible. This research is supported by the National Science Foundation through the AAG program and the XSEDE collaboration, and uses the resources of the Texas Advanced Computing Center.

Scattering Polarization in Solar Flares

Czech Academy of Sciences Publication Activity Database

Štěpán, Jiří; Heinzel, Petr

2013-01-01

Roč. 778, č. 1 (2013), L6/1-L6/6 ISSN 2041-8205 R&D Projects: GA ČR GAP209/12/1652; GA ČR GPP209/12/P741 Institutional support: RVO:67985815 Keywords : line formation * polarization * radiative transfer Subject RIV: BN - Astronomy, Celestial Mechanics, Astrophysics Impact factor: 5.602, year: 2013

One photon exchange processes and the calibration of polarization of high energy protons

International Nuclear Information System (INIS)

Margolis, B.; Thomas, G.H.

1978-01-01

Polarization phenomena in small momentum transfer high energy one-photon exchange processes in the reaction p + A → X + A where A is a complex nucleus and X is anything are examined. It is shown that these polarizations can be related directly to photoproduction polarization effects in the reaction γ + p → X at low energies. Explicit formulae are written for polarization effects in the case where X → π 0 + p

Probing Quark-Gluon Interactions with Transverse Polarized Scattering

International Nuclear Information System (INIS)

Rondon, Oscar A.

2011-01-01

Transverse polarized inelastic scattering extends the power of the electromagnetic interaction as a probe of nucleon dynamics beyond the leading order regime explored with longitudinally polarized DIS. In transverse polarized scattering, the twist-3 g 2 spin structure function contributes at the same order as the longitudinal, twist-2, g 1 , so interactions between quarks and gluons can be studied, opening a window on the mechanisms of confinement. This talk reports the results of Jefferson Lab's Resonances Spin Structure experiment measurement of g 2 and the d 2 twist-3 quark matrix element at a four-momentum transfer of 1.3 GeV 2 .

Manipulating the dipole layer of polar organic molecules on metal surfaces via different charge-transfer channels

Science.gov (United States)

Lin, Meng-Kai; Nakayama, Yasuo; Zhuang, Ying-Jie; Wang, Chin-Yung; Pi, Tun-Wen; Ishii, Hisao; Tang, S.-J.

The key properties of organic films such as energy level alignment (ELA), work functions, and injection barriers are closely linked to this dipole layer. Using angle resolved photoemission spectroscopy (ARPES), we systemically investigate the coverage-dependent work functions and spectra line shapes of occupied molecular orbital states of a polar molecule, chloroaluminium phthalocyanine (ClAlPc), grown on Ag(111) to show that the orientations of the first ClAlPc layer can be manipulated via the molecule deposition rate and post annealing, causing ELA at organic-metal interface to differ for about 0.3 eV between Cl-up and Cl-down configuration. Moreover, by comparing the experimental results with the calculations based on both gas-phase model and realistic model of ClAlPc on Ag(111) , we evidence that the different orientations of ClAlPc dipole layers lead to different charge-transfer channels between ClAlPc and Ag, a key factor that controls the ELA at organic-metal interface.

Elastic proton-deuteron backward scattering: relativistic effects and polarization observables

International Nuclear Information System (INIS)

Kaptari, L.P.; Semikh, S.S.

1997-10-01

The elastic proton-deuteron backward reaction is analyzed within a covariant approach based on the Bethe-Salpeter equation with 000. Lorentz boost and other relativistic effects in the cross section and spin correlation observables, like tensor analyzing power and polarization transfer etc., are investigated in explicit form. Results of numerical calculations for a complete set of polarization observables are presented. (orig.)

Energy transfer in porous anodic alumina/rhodamine 110 nanocomposites

Energy Technology Data Exchange (ETDEWEB)

Elhouichet, H., E-mail: habib.elhouichet@fst.rnu.tn [Laboratoire de Physico-Chimie des Materiaux Mineraux et leurs Applications, Centre National de Recherches en Sciences des Materiaux, B.P. 95, Hammam-Lif 2050 (Tunisia); Departement de Physique, Faculte des Sciences de Tunis, University of Tunis Elmanar 2092 Tunis (Tunisia); Harima, N.; Koyama, H. [Hyogo University of Teacher Education, Kato, Hyogo 673-1494 (Japan); Gaponenko, N.V. [Belarusian State University of Informatics and Radioelectronics, P. Browki St. 6, 220013 Minsk (Belarus)

2012-09-15

We have used porous anodic alumina (PAA) films as templates for embedding rhodamine 110 (Rh110) molecules and examined their photoluminescence (PL) properties in detail. The analysis of the polarization memory (PM) of PL strongly suggests that there is a significant energy transfer from PAA to Rh110 molecules. The effect of annealing the PAA layer on the PL properties of the nanocomposite has been studied. The results show that the energy transfer becomes more efficient in annealed PAA. - Highlights: Black-Right-Pointing-Pointer Porous anodic alumina-rhodamine 110 nanocomposites are elaborated. Black-Right-Pointing-Pointer Efficient energy transfer from the host to Rh110 molecules is evidenced from measurements of photoluminescence and degree of polarization memory spectra. Black-Right-Pointing-Pointer Thermal annealing of porous anodic alumina can improve the process of excitation transfer.

Longitudinal {lambda} and anti {lambda} polarization at the COMPASS experiment

Energy Technology Data Exchange (ETDEWEB)

Kang, Donghee

2007-09-15

At the COMPASS experiment at CERN {lambda} and anti {lambda} particles are produced in deep inelastic scattering (DIS) processes with high statistics. The main focus of the research is the understanding of the spin transfer mechanism from quarks to hadrons through the fragmentation process by utilizing the longitudinal {lambda} and anti {lambda} polarization. The result of the spin transfer provides useful information to test different model predictions which describe spin effects in hyperon production and the quark-antiquark asymmetry of the nucleon and hyperon. The {lambda} and anti {lambda} polarization are determined by measuring the acceptance corrected angular distribution of its decay products. A Monte Carlo simulation is used to correct the acceptance of the COMPASS spectrometer. In this work, preliminary results from data collected in the current fragmentation region during 2002-2004 are presented. A significantly positive average spin transfer of anti {lambda} is found to be equal to C{sub LL}=+0.232{+-}0.039(stat.){+-}0.022(sys.), while the spin transfer of lambda is compatible with zero within the statistical accuracy. The dependences of the spin transfer on various kinematic variables are also presented. (orig.)

Longitudinal Λ and anti Λ polarization at the COMPASS experiment

International Nuclear Information System (INIS)

Kang, Donghee

2007-09-01

At the COMPASS experiment at CERN Λ and anti Λ particles are produced in deep inelastic scattering (DIS) processes with high statistics. The main focus of the research is the understanding of the spin transfer mechanism from quarks to hadrons through the fragmentation process by utilizing the longitudinal Λ and anti Λ polarization. The result of the spin transfer provides useful information to test different model predictions which describe spin effects in hyperon production and the quark-antiquark asymmetry of the nucleon and hyperon. The Λ and anti Λ polarization are determined by measuring the acceptance corrected angular distribution of its decay products. A Monte Carlo simulation is used to correct the acceptance of the COMPASS spectrometer. In this work, preliminary results from data collected in the current fragmentation region during 2002-2004 are presented. A significantly positive average spin transfer of anti Λ is found to be equal to C LL =+0.232±0.039(stat.)±0.022(sys.), while the spin transfer of lambda is compatible with zero within the statistical accuracy. The dependences of the spin transfer on various kinematic variables are also presented. (orig.)

Perturbative determination of c{sub sw} for plaquette and Symanzik gauge action and stout link clover fermions

Energy Technology Data Exchange (ETDEWEB)

Horsley, R. [Edinburgh Univ. (United Kingdom). School of Physics; Perlt, H.; Schiller, A. [Leipzig Univ. (Germany). Inst. fuer Theoretische Physik; Rakow, P.E.L. [Liverpool Univ. (United Kingdom). Theoretical Physics Division, Dept. of Mathematical Sicences; Schierholz, G. [Deutsches Elektronen-Synchrotron (DESY), Hamburg (Germany)

2008-06-15

Using plaquette and Symanzik improved gauge action and stout link clover fermions we determine the improvement coefficient c{sub SW} in one-loop lattice perturbation theory from the off-shell quark-quark-gluon three-point function. In addition, we compute the coefficients needed for the most general form of quark field improvement and present the one-loop result for the critical hopping parameter {kappa}{sub c}. We discuss mean field improvement for c{sub SW} and {kappa}{sub c} and the choice of the mean field coupling for the actions we have considered. (orig.)

Specular, diffuse and polarized imagery of an oat canopy

Science.gov (United States)

Vanderbilt, Vern C.; De Venecia, Kurt J.

1988-01-01

Light, polarized by specular reflection, has been found to be an important part of the light scattered by several measured plant canopies. The authors investigate for one canopy the relative importance of specularly reflected sunlight, specularly reflected light from other sources including skylight, and diffusely upwelling light. Polarization images are used to gain increased understanding of the radiation transfer process in a plant canopy. Analysis of the results suggests that properly analyzed polarized remotely sensed data, acquired under specific atmospheric conditions by a specially designed sensor, potentially provide measures of physiological and morphological states of plants in a canopy.

Radiometric calibration of a polarization-sensitive sensor

International Nuclear Information System (INIS)

Ahmad, S.P.; Markham, B.L.

1992-01-01

The radiometric accuracy of a sensor is adversely affected by scene polarization if its optical system is sensitive to polarization. Tests performed on the reflective bands of the NS001 Thematic Mapper simulator, an aircraft multispectral scanner, show that it is very sensitive to the polarization state of the incoming radiations. For 100 percent linearly polarized light, errors in the measured intensity vary from -40 to +40 percent, depending on the scan angle and spectral band. To estimate polarization-induced errors in the intensity measured at aircraft level, the intensity and polarization of the atmospheric radiances were simulated using a realistic earth-atmosphere radiative transfer model. For the polarization of atmospheric radiances in the solar meridian plane over a vegetated target, intensity errors may range from -10 to + 10 percent. The polarization-induced errors are highest in the shortest NS001 spectral band (0.450-0.525 microns) because of large atmospheric polarizations contributed by Rayleigh particles and small diluting effects caused by the small contributions of weakly polarized radiations coming from aerosols and the surface. Depending on the illumination and view angles, the errors in derived surface reflectance due to the radiance errors can be very large. In particular, for large off-nadir view angles in the forward scattered direction when the sun is low, the relative errors in the derived surface reflectance can be as large as 4 to 5 times the relative error in the radiances. Polarization sensitivity errors cannot be neglected for the shorter wavelengths when the surface reflectance contribution to atmospheric radiances is very small. 40 refs

A Measurement of the neutron electric form factor at very large momentum transfer using polaried electrions scattering from a polarized helium-3 target

Energy Technology Data Exchange (ETDEWEB)

Kelleher, Aidan [College of William and Mary, Williamsburg, VA (United States)

2010-02-01

Knowledge of the electric and magnetic elastic form factors of the nucleon is essential for an understanding of nucleon structure. Of the form factors, the electric form factor of the neutron has been measured over the smallest range in Q² and with the lowest precision. Jefferson Lab experiment 02-013 used a novel new polarized ³ He target to nearly double the range of momentum transfer in which the neutron form factor has been studied and to measure it with much higher precision. Polarized electrons were scattered off this target, and both the scattered electron and neutron were detected. Gⁿ _E was measured to be 0.0242 ± 0.0020(stat) ± 0.0061(sys) and 0.0247 ± 0.0029(stat) ± 0.0031(sys) at Q² = 1.7 and 2.5 GeV² , respectively.

High-Frequency Dynamic Nuclear Polarization in the Nuclear Rotating Frame

DEFF Research Database (Denmark)

Farrar, C. T.; Hall, D. A.; Gerfen, G. J.

2000-01-01

A proton dynamic nuclear polarization (DNP) NMR signal enhancement (ϵ) close to thermal equilibrium, ϵ = 0.89, has been obtained at high field (B0 = 5 T, νepr = 139.5 GHz) using 15 mM trityl radical in a 40:60 water/glycerol frozen solution at 11 K. The electron-nuclear polarization transfer...... is performed in the nuclear rotating frame with microwave irradiation during a nuclear spin-lock pulse. The growth of the signal enhancement is governed by the rotating frame nuclear spin–lattice relaxation time (T1ρ), which is four orders of magnitude shorter than the nuclear spin–lattice relaxation time (T1n......). Due to the rapid polarization transfer in the nuclear rotating frame the experiment can be recycled at a rate of 1/T1ρ and is not limited by the much slower lab frame nuclear spin–lattice relaxation rate (1/T1n). The increased repetition rate allowed in the nuclear rotating frame provides an effective...

A 282 GHz Probe for Dynamic Nuclear Polarization

DEFF Research Database (Denmark)

Rybalko, Oleksandr; Bowen, Sean; Zhurbenko, Vitaliy

Introduction In DNP, microwave irradiation of a sample facilitates the transfer of spin polarization from electrons tonuclei. One of the way to improve the DNP enhancement is to transfer microwave power from the mm-wave source tothe sample more effectively. Several methods and techniques to effic......Introduction In DNP, microwave irradiation of a sample facilitates the transfer of spin polarization from electrons tonuclei. One of the way to improve the DNP enhancement is to transfer microwave power from the mm-wave source tothe sample more effectively. Several methods and techniques......: microwave can with RF coil; the rest of the probe consists of a waveguide, sample tube and coaxial transmission line. The probe is designed to study cylindrical samples with diameter - 9 mm, and height – 2-20 mm. An RF coil which is housed in cylindrical Macor coil form (dielectric with ε=5.64 and tangent δ...... is 0.0025) surrounds the sample. The RF coil has a saddle form and was madeout of two current loops run on opposite sides of a cylinder (in parallel). Material of the coil is copper wire with diameterequal to 0.7 mm. Coil dimensions are: diameter - 13 mm; height - 22.0 mm. The self resonant frequency...

Polarization of stable and radioactive noble gas nuclei by spin exchange with laser pumped alkali atoms

International Nuclear Information System (INIS)

Calaprice, F.; Happer, W.; Schreiber, D.

1984-01-01

The nuclei of noble gases can be strongly polarized by spin exchange with sufficiently dense optically pumped alkali vapors. Only a small fraction of the spin angular momentum of the alkali atoms is transferred to the nuclear spin of the noble gas. Most of the spin angular momentum is lost to translational angular momentum of the alkali and noble gas atoms about each other. For heavy noble gases most of the angular momentum transfer occurs in alkali-noble-gas van der Waals molecules. The transfer efficiency depends on the formation and breakup rates of the van der Waals molecules in the ambient gas. Experimental methods to measure the spin transfer efficiencies have been developed. Nuclei of radioactive noble gases have been polarized by these methods, and the polarization has been detected by observing the anisotropy of the radioactive decay products. Very precise measurements of the magnetic moments of the radioactive nuclei have been made. 12 references, 9 figures

Proton polarimeters for spin transfer experiments

International Nuclear Information System (INIS)

McNaughton, M.W.

1985-01-01

The design and use of proton polarimeters for spin transfer (Wolfenstein parameter) measurements is discussed. Polarimeters are compared with polarized targets for spin dependent experiments. 32 refs., 4 figs

APC: A new code for Atmospheric Polarization Computations

International Nuclear Information System (INIS)

Korkin, Sergey V.; Lyapustin, Alexei I.; Rozanov, Vladimir V.

2013-01-01

A new polarized radiative transfer code Atmospheric Polarization Computations (APC) is described. The code is based on separation of the diffuse light field into anisotropic and smooth (regular) parts. The anisotropic part is computed analytically. The smooth regular part is computed numerically using the discrete ordinates method. Vertical stratification of the atmosphere, common types of bidirectional surface reflection and scattering by spherical particles or spheroids are included. A particular consideration is given to computation of the bidirectional polarization distribution function (BPDF) of the waved ocean surface. -- Highlights: •A new code, APC, has been developed. •The code was validated against well-known codes. •The BPDF for an arbitrary Mueller matrix is computed

Free energy functionals for polarization fluctuations: Pekar factor revisited.

Science.gov (United States)

Dinpajooh, Mohammadhasan; Newton, Marshall D; Matyushov, Dmitry V

2017-02-14

The separation of slow nuclear and fast electronic polarization in problems related to electron mobility in polarizable media was considered by Pekar 70 years ago. Within dielectric continuum models, this separation leads to the Pekar factor in the free energy of solvation by the nuclear degrees of freedom. The main qualitative prediction of Pekar's perspective is a significant, by about a factor of two, drop of the nuclear solvation free energy compared to the total (electronic plus nuclear) free energy of solvation. The Pekar factor enters the solvent reorganization energy of electron transfer reactions and is a significant mechanistic parameter accounting for the solvent effect on electron transfer. Here, we study the separation of the fast and slow polarization modes in polar molecular liquids (polarizable dipolar liquids and polarizable water force fields) without relying on the continuum approximation. We derive the nonlocal free energy functional and use atomistic numerical simulations to obtain nonlocal, reciprocal space electronic and nuclear susceptibilities. A consistent transition to the continuum limit is introduced by extrapolating the results of finite-size numerical simulation to zero wavevector. The continuum nuclear susceptibility extracted from the simulations is numerically close to the Pekar factor. However, we derive a new functionality involving the static and high-frequency dielectric constants. The main distinction of our approach from the traditional theories is found in the solvation free energy due to the nuclear polarization: the anticipated significant drop of its magnitude with increasing liquid polarizability does not occur. The reorganization energy of electron transfer is either nearly constant with increasing the solvent polarizability and the corresponding high-frequency dielectric constant (polarizable dipolar liquids) or actually noticeably increases (polarizable force fields of water).

Free energy functionals for polarization fluctuations: Pekar factor revisited

International Nuclear Information System (INIS)

Dinpajooh, Mohammadhasan; Newton, Marshall D.; Matyushov, Dmitry V.

2017-01-01

The separation of slow nuclear and fast electronic polarization in problems related to electron mobility in polarizable media was considered by Pekar 70 years ago. This separation leads to the Pekar factor in the free energy of solvation by the nuclear degrees of freedom, within dielectric continuum models. The main qualitative prediction of Pekar’s perspective is a significant, by about a factor of two, drop of the nuclear solvation free energy compared to the total (electronic plus nuclear) free energy of solvation. The Pekar factor enters the solvent reorganization energy of electron transfer reactions and is a significant mechanistic parameter accounting for the solvent effect on electron transfer. We study the separation of the fast and slow polarization modes in polar molecular liquids (polarizable dipolar liquids and polarizable water force fields) without relying on the continuum approximation. We derive the nonlocal free energy functional and use atomistic numerical simulations to obtain nonlocal, reciprocal space electronic and nuclear susceptibilities. A consistent transition to the continuum limit is introduced by extrapolating the results of finite-size numerical simulation to zero wavevector. The continuum nuclear susceptibility extracted from the simulations is numerically close to the Pekar factor. But, we derive a new functionality involving the static and high-frequency dielectric constants. The main distinction of our approach from the traditional theories is found in the solvation free energy due to the nuclear polarization: the anticipated significant drop of its magnitude with increasing liquid polarizability does not occur. The reorganization energy of electron transfer is either nearly constant with increasing the solvent polarizability and the corresponding high-frequency dielectric constant (polarizable dipolar liquids) or actually noticeably increases (polarizable force fields of water).

Polarization of the sigma minus hyperon produced by a polarized neutral particle beam

International Nuclear Information System (INIS)

Nguyen, A.N.

1992-01-01

A spin transfer technique has been tried in an attempt to produce a beam of polarized hyperons. The method makes use of a two-stage targeting scheme where unpolarized protons from Fermilab's Tevatron incident on target number one (Cu) at production angles of ±2.0 mrad would produce a beam of particles containing polarized Λs and Ξs as well as neutrons and Ks. This secondary beam would then be swept magnetically to retain only neutral particles and brought to bear on target number two (Cu) at 0.0 mrad, producing a tertiary beam of hyperons. The polarization of some 1.3 millions reconstructed Σ - → nπ - events in this tertiary beam (the Σ - having been produced in the inclusive reaction neutrals + Cu → Σ - + X) has been measured at average Σ - momenta 320 GeV/c (1.14 millions events) and 410 GeV/c (135,000 events) and found to be |P| = 3.9 ± 3.2 ± 1.8% and |P| = 13.9 ± 8.1 ± 2.0% respectively, where the first uncertainty is statistical and the second systematic. These polarizations are small and consistent with zero, and preclude a meaningful measurement of the Σ - magnetic moment by the spin precession method. The sign of the polarizations at the target is ambiguous, giving rise to two possible different solutions for the magnetic moment-one of two possible different solutions for the magnetic moment-one of which distinctly disagrees with the world average value for the moment. However, this solution fits the data slightly better than the other. This inconsistency would not exist if the polarization is, in fact, zero

Magnetic systems for wide-aperture neutron polarizers and analyzers

Energy Technology Data Exchange (ETDEWEB)

Gilev, A.G. [Neutron Research Department, Petersburg Nuclear Physics Institute, NRC “Kurchatov Institute”, Orlova Roscha, Gatchina, St. Petersburg 188300 (Russian Federation); Pleshanov, N.K., E-mail: pnk@pnpi.spb.ru [Neutron Research Department, Petersburg Nuclear Physics Institute, NRC “Kurchatov Institute”, Orlova Roscha, Gatchina, St. Petersburg 188300 (Russian Federation); Bazarov, B.A.; Bulkin, A.P.; Schebetov, A.F. [Neutron Research Department, Petersburg Nuclear Physics Institute, NRC “Kurchatov Institute”, Orlova Roscha, Gatchina, St. Petersburg 188300 (Russian Federation); Syromyatnikov, V.G. [Neutron Research Department, Petersburg Nuclear Physics Institute, NRC “Kurchatov Institute”, Orlova Roscha, Gatchina, St. Petersburg 188300 (Russian Federation); Physical Department, St. Petersburg State University, Ulyanovskaya, 1, Petrodvorets, St. Petersburg 198504 (Russian Federation); Tarnavich, V.V.; Ulyanov, V.A. [Neutron Research Department, Petersburg Nuclear Physics Institute, NRC “Kurchatov Institute”, Orlova Roscha, Gatchina, St. Petersburg 188300 (Russian Federation)

2016-10-11

Requirements on the field uniformity in neutron polarizers are analyzed in view of the fact that neutron polarizing coatings have been improved during the past decade. The design of magnetic systems that meet new requirements is optimized by numerical simulations. Magnetic systems for wide-aperture multichannel polarizers and analyzers are represented, including (a) the polarizer to be built at channel 4-4′ of the reactor PIK (Gatchina, Russia) for high-flux experiments with a 100×150 mm{sup 2} beam of polarized cold neutrons; (b) the fan analyzer covering a 150×100 mm{sup 2} window of the detector at the Magnetism Reflectometer (SNS, ORNL, USA); (c) the polarizer and (d) the fan analyzer covering a 220×110 mm{sup 2} window of the detector at the reflectometer NERO, which is transferred to PNPI (Russia) from HZG (Germany). Deviations of the field from the vertical did not exceed 2°. The polarizing efficiency of the analyzer at the Magnetism Reflectometer reached 99%, a record level for wide-aperture supermirror analyzers.

Polarization Switching and Light-Enhanced Piezoelectricity in Lead Halide Perovskites.

Science.gov (United States)

Coll, Mariona; Gomez, Andrés; Mas-Marza, Elena; Almora, Osbel; Garcia-Belmonte, Germà; Campoy-Quiles, Mariano; Bisquert, Juan

2015-04-16

We investigate the ferroelectric properties of photovoltaic methylammonium lead halide CH3NH3PbI3 perovskite using piezoelectric force microscopy (PFM) and macroscopic polarization methods. The electric polarization is clearly observed by amplitude and phase hysteresis loops. However, the polarization loop decreases as the frequency is lowered, persisting for a short time only, in the one second regime, indicating that CH3NH3PbI3 does not exhibit permanent polarization at room temperature. This result is confirmed by macroscopic polarization measurement based on a standard capacitive method. We have observed a strong increase of piezoelectric response under illumination, consistent with the previously reported giant photoinduced dielectric constant at low frequencies. We speculate that an intrinsic charge transfer photoinduced dipole in the perovskite cage may lie at the origin of this effect.

Spin-polarization reversal at the interface between benzene and Fe(100)

KAUST Repository

Goumri-Said, Souraya

2013-01-03

The spin-polarization at the interface between Fe(100) and a benzene is investigated theoretically using density functional theory for two positions of the organic molecule: planar and perpendicular with respect to the substrate. The electronic and magnetic properties as well as the spin-polarization close to the Fermi level strongly depend on the benzene position on the iron surface. An inversion of the spin-polarization is induced by p-d hybridization and charge transfer from the iron to the carbon sites in both configurations.

Spin-polarization reversal at the interface between benzene and Fe(100)

KAUST Repository

Goumri-Said, Souraya; Benali Kanoun, Mohammed; Manchon, Aurelien; Schwingenschlö gl, Udo

2013-01-01

The spin-polarization at the interface between Fe(100) and a benzene is investigated theoretically using density functional theory for two positions of the organic molecule: planar and perpendicular with respect to the substrate. The electronic and magnetic properties as well as the spin-polarization close to the Fermi level strongly depend on the benzene position on the iron surface. An inversion of the spin-polarization is induced by p-d hybridization and charge transfer from the iron to the carbon sites in both configurations.

Exploiting level anti-crossings for efficient and selective transfer of hyperpolarization in coupled nuclear spin systems

NARCIS (Netherlands)

Pravdivtsev, A.N.; Yurkovskaya, A.V.; Kaptein, R.; Miesel, K.; Vieth, H.-M.; Ivanov, K.L.

2013-01-01

Spin hyperpolarization can be coherently transferred to other nuclei in field-cycling NMR experiments. At low magnetic fields spin polarization is redistributed in a strongly coupled network of spins. Polarization transfer is most efficient at fields where level anti-crossings (LACs) occur for the

Nuclear spin polarization of targets

International Nuclear Information System (INIS)

Happer, W.

1990-01-01

Lasers can be used to produce milligrams to grams of noble gas nuclei with spin polarizations in excess of 50%. These quantities are sufficient to be very useful targets in nuclear physics experiments. Alkali-metal atoms are used to capture the angular momentum of circularly polarized laser photons, and the alkali-metal atoms transfer their angular momentum to noble gas atoms in binary or three-body collisions. Non-radiative collisions between the excited alkali atoms and molecular quenching gases are essential to avoid radiation trapping. The spin exchange can involve gas-phase van der Waals molecules, consisting of a noble gas atom and an alkali metal atom. Surface chemistry is also of great importance in determining the wall-induced relaxation rates of the noble gases

From Dark to Light to Fluorescence Resonance Energy Transfer (FRET): Polarity-Sensitive Aggregation-Induced Emission (AIE)-Active Tetraphenylethene-Fused BODIPY Dyes with a Very Large Pseudo-Stokes Shift.

Science.gov (United States)

Şen, Esra; Meral, Kadem; Atılgan, Serdar

2016-01-11

The work presented herein is devoted to the fabrication of large Stokes shift dyes in both organic and aqueous media by combining dark resonance energy transfer (DRET) and fluorescence resonance energy transfer (FRET) in one donor-acceptor system. In this respect, a series of donor-acceptor architectures of 4,4-difluoro-4-bora-3a,4a-diaza-s-indacene (BODIPY) dyes substituted by one, two, or three tetraphenylethene (TPE) luminogens were designed and synthesised. The photophysical properties of these three chromophore systems were studied to provide insight into the nature of donor-acceptor interactions in both THF and aqueous media. Because the generation of emissive TPE donor(s) is strongly polarity dependent, due to its aggregation-induced emission (AIE) feature, one might expect the formation of appreciable fluorescence emission intensity with a very large pseudo-Stokes shift in aqueous media when considering FRET process. Interestingly, similar results were also recorded in THF for the chromophore systems, although the TPE fragment(s) of the dyes are non-emissive. The explanation for this photophysical behaviour lies in the DRET. This is the first report on combining two energy-transfer processes, namely, FRET and DRET, in one polarity-sensitive donor-acceptor pair system. The accuracy of the dark-emissive donor property of the TPE luminogen is also presented for the first time as a new feature for AIE phenomena. © 2016 WILEY-VCH Verlag GmbH & Co. KGaA, Weinheim.

Light scattering reviews 8 radiative transfer and light scattering

CERN Document Server

Kokhanovsky, Alexander A

2013-01-01

Light scattering review (vol 8) is aimed at the presentation of recent advances in radiative transfer and light scattering optics. The topics to be covered include: scattering of light by irregularly shaped particles suspended in atmosphere (dust, ice crystals), light scattering by particles much larger as compared the wavelength of incident radiation, atmospheric radiative forcing, astrophysical radiative transfer, radiative transfer and optical imaging in biological media, radiative transfer of polarized light, numerical aspects of radiative transfer.

Study of the proton structure by measurements of polarization transfers in real Compton scattering at J Lab

International Nuclear Information System (INIS)

Fanelli, C.; Salme, G.; Cisbani, E.; Hamilton, D.; Wojtsekhowski, B.

2014-01-01

A preliminary analysis of polarization-transfer data at large scattering angle (70 degrees), obtained in an experiment of real Compton scattering on proton, performed in Hall-C of Jefferson Lab, is presented. It is also discussed the relevance of this kind of experiments for shedding light on the non-perturbative structure of the proton, at low energy, and on the transition from the non-perturbative regime to the perturbative one, that occurs at high energy. Moreover, the possibility to extract Compton form factors and the Generalized Parton Distributions (GPD), one of the most promising theoretical tool to determine the total angular momentum contribution of quarks and gluons to nucleon spin, is emphasized. The preliminary results appear consistent with GPD's based and Regge predictions. This is not sufficient yet to exclude pQCD COZ (Chernyak-Oglobin-Zhitnistsky) model, but it is another preliminary indication that the handbag approach seems to be the dominant mechanism at the energy of the experiment

Investigation of PTFE transfer films by infrared emission spectroscopy and phase-locked ellipsometry

Science.gov (United States)

Lauer, James L.; Bunting, Bruce G.; Jones, William R., Jr.

1988-01-01

When a PTFE sheet was rubbed unidirectionally over a smooth surface of stainless steel an essentially monomolecular transfer film was formed. by ellipsometric and emission infrared spectroscopic techniques it was shown that the film was 10 to 15 A thick and birefringent. From the intensity differences of infrared bands obtained with a polarizer passing radiation polarized in mutually perpendicular planes, it was possible to deduce transfer film orientation with the direction of rubbing. After standing in air for several weeks the transfer films apparently increased in thickness by as much as threefold. At the same time both the index of refraction and the absorption index decreased. Examination of the surfaces by optical and electron microscopies showed that the films had become porous and flaky. These observations were consistent with previous tribological measurements. The coefficients of friction decreased with the formation of the transfer film but increased again as the film developed breaks. The applicability of the ellipsometric and polarized infrared emission techniques to the identification of monomolecular tribological transfer films of polymers such as PTFE has been demonstrated.

Development of high-polarization Fe/Ge neutron polarizing supermirror: Possibility of fine-tuning of scattering length density in ion beam sputtering

Science.gov (United States)

Maruyama, R.; Yamazaki, D.; Akutsu, K.; Hanashima, T.; Miyata, N.; Aoki, H.; Takeda, M.; Soyama, K.

2018-04-01

The multilayer structure of Fe/Si and Fe/Ge systems fabricated by ion beam sputtering (IBS) was investigated using X-ray and polarized neutron reflectivity measurements and scanning transmission electron microscopy with energy-dispersive X-ray analysis. The obtained result revealed that the incorporation of sputtering gas particles (Ar) in the Ge layer gives rise to a marked reduction in the neutron scattering length density (SLD) and contributes to the SLD contrast between the Fe and Ge layers almost vanishing for spin-down neutrons. Bundesmann et al. (2015) have shown that the implantation of primary Ar ions backscattered at the target is responsible for the incorporation of Ar particles and that the fraction increases with increasing ion incidence angle and increasing polar emission angle. This leads to a possibility of fine-tuning of the SLD for the IBS, which is required to realize a high polarization efficiency of a neutron polarizing supermirror. Fe/Ge polarizing supermirror with m = 5 fabricated under the same condition showed a spin-up reflectivity of 0.70 at the critical momentum transfer. The polarization was higher than 0.985 for the qz range where the correction for the polarization inefficiencies of the beamline works properly. The result of the polarized neutron reflectivity measurement suggests that the "magnetically-dead" layers formed at both sides of the Fe layer, together with the SLD contrast, play a critical role in determining the polarization performance of a polarizing supermirror.

COST meeting - Polarization and AGN II - Abstracts and slides

International Nuclear Information System (INIS)

Kishimoto, M.; Rouan, D.; Tadhunter, C.; Lopez Rodriguez, E.; Braibant, L.; Pasetto, A.; Matt, G.; Afanasiev, V.; Lira, P.; Hutsemekers, D.; Sluse, D.; Marin, F.; Tamborra, F.; Yankova, K.; Laing, R.; Lico, R.; Agudo, I.; Hovatta, T.; Jermak, H.; Chen, X.; Myserlis, I.; Cellone, S.A.; Chidiac, C.; Chakraborty, N.; Bozhilov, V.

2016-01-01

This meeting is the 2. COST workshop on Polarization and Active Galactic Nuclei (AGN). Accreting supermassive black holes in active galactic nuclei are the most powerful, long-lasting sources in the universe. Emitting over ten orders of magnitude in photon energy or more, the radiation of AGN encodes information about a multitude of astrophysical processes: accretion, thermal and non-thermal radiative transfer, acceleration of outflows and jets, shock physics, special and general relativity. Observationally, AGN appear as numerous types and polarization studies have played a key role in establishing the idea of a unifying AGN geometry. The topics covered at the meeting include the following: 1) Polarimetry of AGN from the radio to gamma-rays; 2) Tools for modeling and data analysis of AGN polarization; 3) Polarization due to magnetic fields and dust in AGN; 4) Polarization of AGN inflows, outflows and jets; 5) Spectropolarimetry and polarization variability of AGN; and 6) From Sgr A* to the most luminous quasars: what can polarimetry do for AGN (super-)unification? This document is made up of the abstracts and slides of the presentations

Measurement of spin-transfer observables in pp to $\\Lambda \\Lambda$ at 1.637 GeV/c

CERN Document Server

Bassalleck, B; Bradtke, C; Bröders, R; Bunker, B; Dennert, H; Dutz, H; Eilerts, S W; Eyrich, W; Fields, D; Fischer, H; Franklin, G; Franz, J; Gehring, R; Geyer, R; Görtz, S; Harmsen, J; Hauffe, J; Heinsius, F H; Hertzog, D W; Johansson, T; Jones, T; Khaustov, P; Kilian, K; Kingsberry, P; Kriegler, E; Lowe, J; Meier, A; Metzger, A E; Meyer, C A; Meyer, Werner T; Moosburger, M; Oelert, W; Paschke, K D; Plückthun, M; Pomp, S; Quinn, B; Radtke, E; Reicherz, G; Röhrich, K; Sachs, K; Schmitt, H; Schoch, B; Sefzick, T; Stinzing, F; Stotzer, R W; Tayloe, R; Wirth, S

2002-01-01

Spin-transfer observables for pp to Lambda Lambda have been measured using a transversely polarized frozen-spin target and a beam momentum of 1.637 GeV/c. Current models of the reaction near threshold are in good agreement with existing measurements performed with unpolarized particles in the initial state but produce conflicting predictions for the spin-transfer observables D/sub nn/ and K/sub nn/ (the normal-to-normal depolarization and polarization transfer), which are measurable only with polarized target or beam. Measurements of D/sub nn/ and K/sub nn/ presented here are found to be in disagreement with predictions from these models. (21 refs).

Polarization Study for NLC Positron Source Using EGS4

Energy Technology Data Exchange (ETDEWEB)

Liu, James C

2000-09-20

SLAC is exploring a polarized positron source to study new physics for the NLC project. The positron source envisioned in this paper consists of a polarized electron source, a 50-MeV electron accelerator, a thin target less-than-or-equal-to 0.2 radiation length for positron production, and a capture system for high-energy, small angular divergence positrons. The EGS4 code was used to study the yield, energy spectra, emission-angle distribution, and the mean polarization of the positrons emanating from W-Re and Ti targets hit by longitudinally polarized electron and photon beams. To account for polarization within the EGS4 code a method devised by Flottmann was used, which takes into account polarization transfer for pair production, bremsstrahlung, and Compton interactions. A mean polarization of 0.85 for positrons with energies greater than 25 MeV was obtained. Most of the high-energy positrons were emitted within a forward angle of 20 degrees. The yield of positrons above 25 MeV per incident photon was 0.034, which was about 70 times higher than that obtained with an electron beam.

Proton polarizing system with Ar-ion laser for p-vector-RI scattering experiments

International Nuclear Information System (INIS)

Wakui, T.; Hatano, M.; Sakai, H.; Uesaka, T.; Tamii, A.

2005-01-01

A proton polarizing system for use in scattering experiments with radioactive isotope beams is described. Protons in a naphthalene crystal doped with pentacene are polarized in a magnetic field of 0.3T at 100K by transferring a large population difference among the photo-excited triplet states of pentacene to the hydrogen nuclei. An Ar-ion laser, which demands minimal maintenance during scattering experiments, is employed to excite the pentacene molecules. A proton polarization of 37% is obtained

Quantum theory of nonadiabatic heavy-particle transfer processes in polar media

International Nuclear Information System (INIS)

Kuznetsov, A.M.

1986-01-01

For the probability of nonadiabatic transfer of heavy particles, a calculating procedure is proposed which in the case of certain processes allows the interaction between motion of the particle undergoing transfer and motion along other degrees of freedom to be exactly accounted for. In the case of symmetric systems, explicit expressions are obtained for the free energy of activation of the transition and for the tunneling factor which allow for nonadiabaticity of motion of the particle undergoing transfer, both in the region beneath the barrier and in the region that is classically accessible

Measurement of K/sub NN/, K/sub SS/, K/sub SL/, and K/sub LL/ in polarized np → polarized pn at 800 MeV in the CEX region

International Nuclear Information System (INIS)

Ransome, R.D.; Hollas, C.L.; Riley, P.J.

1980-01-01

The spin transfer parameters K/sub NN/, K/sub SS/, K/sub SL/, and K/sub LL/ have been measured for np elastic scattering at 800 MeV between 165 0 and 180 0 c.m. The parameters K/sub NN/ and K/sub LL/ are in good agreement with the quasi-free reaction polarized pd → polarized npp at 180 0

Quantitative determination of high-Tc superconductivity from the lattice polarization, structure effect and approach to 300 K Tc

International Nuclear Information System (INIS)

Green, B.A.

1997-01-01

The quasiparticle state defined by the low temperature polar mobility is a large, quantized positive energy shift that is identical to the constant pairing energy (pseudogap and 2Λ) in the multi-plane high-T c superconductors, showing the lattice polarization produces the single-particle shift and pairing which then transfer to the superconducting state. The coupling-independence and state transfer follow from the nonlocality and action length of the polarization interaction, and the multiple plane requirement from the location of the polar mode. 2Δ is thereby obtained directly, without scaling, from the strong interaction on the plane. The interaction accordingly produces a dynamic, highly stable state, in contrast to BCS superconductors, and the zero-order state is the quantized energy shift. (orig.)

Probing energy transfer events in the light harvesting complex 2 (LH2) of Rhodobacter sphaeroides with two-dimensional spectroscopy.

Science.gov (United States)

Fidler, Andrew F; Singh, Ved P; Long, Phillip D; Dahlberg, Peter D; Engel, Gregory S

2013-10-21

Excitation energy transfer events in the photosynthetic light harvesting complex 2 (LH2) of Rhodobacter sphaeroides are investigated with polarization controlled two-dimensional electronic spectroscopy. A spectrally broadened pulse allows simultaneous measurement of the energy transfer within and between the two absorption bands at 800 nm and 850 nm. The phased all-parallel polarization two-dimensional spectra resolve the initial events of energy transfer by separating the intra-band and inter-band relaxation processes across the two-dimensional map. The internal dynamics of the 800 nm region of the spectra are resolved as a cross peak that grows in on an ultrafast time scale, reflecting energy transfer between higher lying excitations of the B850 chromophores into the B800 states. We utilize a polarization sequence designed to highlight the initial excited state dynamics which uncovers an ultrafast transfer component between the two bands that was not observed in the all-parallel polarization data. We attribute the ultrafast transfer component to energy transfer from higher energy exciton states to lower energy states of the strongly coupled B850 chromophores. Connecting the spectroscopic signature to the molecular structure, we reveal multiple relaxation pathways including a cyclic transfer of energy between the two rings of the complex.

Probing energy transfer events in the light harvesting complex 2 (LH2) of Rhodobacter sphaeroides with two-dimensional spectroscopy

Energy Technology Data Exchange (ETDEWEB)

Fidler, Andrew F.; Singh, Ved P.; Engel, Gregory S. [Department of Chemistry, The Institute for Biophysical Dynamics, and The James Franck Institute, The University of Chicago, Chicago, Illinois 60637 (United States); Long, Phillip D.; Dahlberg, Peter D. [Graduate Program in the Biophysical Sciences, The University of Chicago, Chicago, Illinois 60637 (United States)

2013-10-21

Excitation energy transfer events in the photosynthetic light harvesting complex 2 (LH2) of Rhodobacter sphaeroides are investigated with polarization controlled two-dimensional electronic spectroscopy. A spectrally broadened pulse allows simultaneous measurement of the energy transfer within and between the two absorption bands at 800 nm and 850 nm. The phased all-parallel polarization two-dimensional spectra resolve the initial events of energy transfer by separating the intra-band and inter-band relaxation processes across the two-dimensional map. The internal dynamics of the 800 nm region of the spectra are resolved as a cross peak that grows in on an ultrafast time scale, reflecting energy transfer between higher lying excitations of the B850 chromophores into the B800 states. We utilize a polarization sequence designed to highlight the initial excited state dynamics which uncovers an ultrafast transfer component between the two bands that was not observed in the all-parallel polarization data. We attribute the ultrafast transfer component to energy transfer from higher energy exciton states to lower energy states of the strongly coupled B850 chromophores. Connecting the spectroscopic signature to the molecular structure, we reveal multiple relaxation pathways including a cyclic transfer of energy between the two rings of the complex.

Probing energy transfer events in the light harvesting complex 2 (LH2) of Rhodobacter sphaeroides with two-dimensional spectroscopy

International Nuclear Information System (INIS)

Fidler, Andrew F.; Singh, Ved P.; Engel, Gregory S.; Long, Phillip D.; Dahlberg, Peter D.

2013-01-01

Excitation energy transfer events in the photosynthetic light harvesting complex 2 (LH2) of Rhodobacter sphaeroides are investigated with polarization controlled two-dimensional electronic spectroscopy. A spectrally broadened pulse allows simultaneous measurement of the energy transfer within and between the two absorption bands at 800 nm and 850 nm. The phased all-parallel polarization two-dimensional spectra resolve the initial events of energy transfer by separating the intra-band and inter-band relaxation processes across the two-dimensional map. The internal dynamics of the 800 nm region of the spectra are resolved as a cross peak that grows in on an ultrafast time scale, reflecting energy transfer between higher lying excitations of the B850 chromophores into the B800 states. We utilize a polarization sequence designed to highlight the initial excited state dynamics which uncovers an ultrafast transfer component between the two bands that was not observed in the all-parallel polarization data. We attribute the ultrafast transfer component to energy transfer from higher energy exciton states to lower energy states of the strongly coupled B850 chromophores. Connecting the spectroscopic signature to the molecular structure, we reveal multiple relaxation pathways including a cyclic transfer of energy between the two rings of the complex

Li breakup polarization potential at near barrier energies

International Nuclear Information System (INIS)

Lubian, F. J.; Correa, T.; Gomes, P.R.S.; Paes, B; Figueira, J. M.; Abriola, D.; Fernandez, J. O.; Capurro, O. A.; Marti, G.V.; Martinez, D.; Heimann; Negri, A.; Pacheco, A. J.; Padron, I.

2007-01-01

Inelastic and one neutron transfer cross sections at energies around the Coulomb barrier were used to derive dynamic polarization potential (DPP) for the 7 Li + 27 Al system. The DPP due to breakup, obtained in a simple way, indicates that its real part is repulsive at nearbarrier energies. (Author)

On some methods to produce high-energy polarized electron beams by means of proton synchrotrons

International Nuclear Information System (INIS)

Bessonov, E.G.; Vazdik, Ya.A.

1980-01-01

Some methods of production of high-energy polarized electron beams by means of proton synchrotrons are considered. These methods are based on transfer by protons of a part of their energy to the polarized electrons of a thin target placed inside the working volume of the synchrotron. It is suggested to use as a polarized electron target a magnetized crystalline iron in which proton channeling is realized, polarized atomic beams and the polarized plasma. It is shown that by this method one can produce polarized electron beams with energy approximately 100 GeV, energy spread +- 5 % and intensity approximately 10 7 electron/c, polarization approximately 30% and with intensity approximately 10 4 -10 5 electron/c, polarization approximately 100% [ru

Proton-transfer reactions in ionized gases

International Nuclear Information System (INIS)

Stiller, W.; Schmidt, R.; Schuster, R.

1985-01-01

Ion-molecule reactions play an important role in various radiolytic processes, e.g. gas-pulse radiolysis, environmental research. For a discussion of mechanisms rate coefficients have to be assessed. Here gas-phase rate coefficients of ion-(polar) molecule reactions are calculated using the ideas of interaction potentials, reactive cross-sections and distribution functions of the translational energies of both the reactants (ions I, molecules M). The starting point of our approach, directed especially to gas-phase proton-transfer reactions, is the idea that the rate coefficient k can be calculated as an ion-molecule capture-rate coefficient multiplied by a 'steric factor' representing the probability for proton transfer. Mutual capture of the reaction partners within a possible reaction zone is caused by the physical interaction between an ion and a polar molecule. A model is discussed. Results are presented. (author)

Selective Deflection of Polarized Light Via Coherently Driven Four-Level Atoms in a Double-Λ Configuration

International Nuclear Information System (INIS)

Guo Yu

2010-01-01

We study the interaction of a weak probe field, having two circular polarized components, i.e., σ - and σ + polarization, with an optically dense medium of four-level atoms in a double-Λ configuration, which is mediated by the electromagnetically induced transparency with a polarized control light with spatially inhomogeneous profile. We analyse the deflection of the polarized probe light and we find that we can selectively determine which circular component will be deflected after the polarized probe light enters the atom medium via adjusting the polarization and detuning of the control field. (electromagnetism, optics, acoustics, heat transfer, classical mechanics, and fluid dynamics)

Molecular electron recollision dynamics in intense circularly polarized laser pulses

Science.gov (United States)

Bandrauk, André D.; Yuan, Kai-Jun

2018-04-01

Extreme UV and x-ray table top light sources based on high-order harmonic generation (HHG) are focused now on circular polarization for the generation of circularly polarized attosecond pulses as new tools for controlling electron dynamics, such as charge transfer and migration and the generation of attosecond quantum electron currents for ultrafast magneto-optics. A fundamental electron dynamical process in HHG is laser induced electron recollision with the parent ion, well established theoretically and experimentally for linear polarization. We discuss molecular electron recollision dynamics in circular polarization by theoretical analysis and numerical simulation. The control of the polarization of HHG with circularly polarized ionizing pulses is examined and it is shown that bichromatic circularly polarized pulses enhance recollision dynamics, rendering HHG more efficient, especially in molecules because of their nonspherical symmetry. The polarization of the harmonics is found to be dependent on the compatibility of the rotational symmetry of the net electric field created by combinations of bichromatic circularly polarized pulses with the dynamical symmetry of molecules. We show how the field and molecule symmetry influences the electron recollision trajectories by a time-frequency analysis of harmonics. The results, in principle, offer new unique controllable tools in the study of attosecond molecular electron dynamics.

Fractal structure of hadrons in processes with polarized protons at SPD NICA (proposal for experiment)

International Nuclear Information System (INIS)

Tokarev, M.V.; Aparin, A.A.; Zborovsky, I.

2014-01-01

The concept of z-scaling previously developed for analysis of inclusive reactions in proton-proton collisions is applied for description of processes with polarized protons at the planned Spin Physics Detector NICA in Dubna. A hypothesis of self-similarity and fractality of the proton spin structure is discussed. The possibilities to extract information on spin-dependent fractal dimensions of hadrons and fragmentation process from asymmetries and coefficients of polarization transfer are justified. The double longitudinal spin asymmetry A LL of π 0 -meson production and the coefficient of the polarization transfer D LL of Λ hyperon production in proton-proton collisions measured at RHIC are analyzed in the framework of z-scaling. The spin-dependent fractal dimensions of proton and fragmentation process with polarized Λ hyperon are estimated. A study of the spin-dependent constituent energy loss as a function of transverse momentum of the inclusive hadron and collision energy is suggested.

Redox potentials of free radicals. III. Reevaluation of the method

International Nuclear Information System (INIS)

Rao, P.S.; Hayon, E.

1974-01-01

A reevaluation of the method described in ref 1 and 2 to determine the redox potentials of free radicals (.RH) in water using the techniques of pulse radiolysis and absorption spectrophotometry is presented. This method is based on the dependence of the percentage efficiency for the one-electron oxidation (or reduction) of .RH radicals on the redox potentials E 01 of the electron acceptors, A. The reaction .RH + A → .A - + R + H + (kappa/sub ox/) is not reversible for most radicals under the experimental conditions used, and the derived potentials are, therefore, not thermodynamic values. A reinterpretation of the results is made on the basis of the kinetic competition between the above reaction and .RH + A → .RHA (kappa/sub add/) (radical adducts). Based on kappa/ sub ox/ and kappa/sub add/, it is concluded that the observed experimental ''titration'' curves do represent a measure of the redox property of the free radicals. From the midpoint on the curves, the kinetic potential, E/sub kappa/ 01 : of the free radicals can be derived based on the known two-electron redox potentials of the electron acceptors. These and other questions are discussed. (U.S.)

Many-body kinetics of dynamic nuclear polarization by the cross effect

Science.gov (United States)

Karabanov, A.; Wiśniewski, D.; Raimondi, F.; Lesanovsky, I.; Köckenberger, W.

2018-03-01

Dynamic nuclear polarization (DNP) is an out-of-equilibrium method for generating nonthermal spin polarization which provides large signal enhancements in modern diagnostic methods based on nuclear magnetic resonance. A particular instance is cross-effect DNP, which involves the interaction of two coupled electrons with the nuclear spin ensemble. Here we develop a theory for this important DNP mechanism and show that the nonequilibrium nuclear polarization buildup is effectively driven by three-body incoherent Markovian dissipative processes involving simultaneous state changes of two electrons and one nucleus. We identify different parameter regimes for effective polarization transfer and discuss under which conditions the polarization dynamics can be simulated by classical kinetic Monte Carlo methods. Our theoretical approach allows simulations of the polarization dynamics on an individual spin level for ensembles consisting of hundreds of nuclear spins. The insight obtained by these simulations can be used to find optimal experimental conditions for cross-effect DNP and to design tailored radical systems that provide optimal DNP efficiency.

Evidence for shallow positron traps in a neutron-irradiated Al single crystal

International Nuclear Information System (INIS)

Schultz, P.J.; MacKenzie, I.K.; Lynn, K.G.; West, R.N.; Snead, C.L. Jr.

1982-01-01

Variable energy positrons have been used to determine the dependence on temperature of positron diffusion out of a neutron-irradiated single crystal of Al. The results are interpreted in the context of a one-dimensional diffusion model which includes bulk annihilations as well as trapping at voids and other microstructural defects in the bulk material by way of a removal rate kappa/sub eff/ of freely diffusing positrons. The data show a strongly negative dependence on temperature below 125 0 K for kappa/sub eff/, indicating the presence of some additional phenomenon which we attribute to positron localization in shallow, presumably radiation-induced, traps in the crystal

Excellent polarization-independent reflector based on guided mode resonance effect

International Nuclear Information System (INIS)

Xu Cheng; Xu Lin-Min; Qiang Ying-Huai; Zhu Ya-Bo; Liu Jiong-Tian; Ma Jian-Yong

2011-01-01

A broad band polarization-independent reflector working in the telecommunication C+L band is proposed using the guided mode resonance effect of a periodic surface relief element deposited by a layer of silicon medium. It is shown that this structure can provide high reflection (R > 99.5%) and wide angular bandwidth (θ ≈ 20°, R > 98%) for both TE and TM polarizations over a wide spectrum band 1.5 μm∼1.6 μm. Furthermore, it is found by rigorous coupled wave analysis that the polarization-independent reflector proposed here is tolerant of a deviation of grating thickness, which makes it very easy to fabricate in experiments. (electromagnetism, optics, acoustics, heat transfer, classical mechanics, and fluid dynamics)

Measuring c-quark polarization in W+c samples at ATLAS and CMS

CERN Document Server

Kats, Yevgeny

2016-01-01

The process $pp \\to W^-c$ produces polarized charm quarks. The polarization is expected to be partly retained in $\\Lambda_c$ baryons when those form in the $c$-quark hadronization. We argue that it will likely be possible for ATLAS and CMS to measure the $\\Lambda_c$ polarization in the $W$+$c$ samples in Run 2 of the LHC. This can become the first measurement ever of a longitudinal polarization of charm quarks. Its results will provide a unique input to the understanding of polarization transfer in fragmentation. They will also allow applying the same measurement technique to other (e.g., new physics) samples of charm quarks in which the polarization is a priori unknown. The proposed analysis is similar to the ATLAS and CMS measurements of the $W$+$c$ cross section in the 7 TeV run that used reconstructed $D$-meson decays for charm tagging.

Measuring the influence of aerosols and albedo on sky polarization.

Science.gov (United States)

Kreuter, A; Emde, C; Blumthaler, M

2010-11-01

All-sky distributions of the polarized radiance are measured using an automated fish-eye camera system with a rotating polarizer. For a large range of aerosol and surface albedo situations, the influence on the degree of polarization and sky radiance is investigated. The range of aerosol optical depth and albedo is 0.05-0.5 and 0.1-0.75, respectively. For this range of parameters, a reduction of the degree of polarization from about 0.7 to 0.4 was observed. The analysis is done for 90° scattering angle in the principal plane under clear sky conditions for a broadband channel of 450 ± 25 nm and solar zenith angles between 55° and 60°. Radiative transfer calculations considering three different aerosol mixtures are performed and and agree with the measurements within the statistical error.

Oxygen ion transference number of doped lanthanum gallate

Science.gov (United States)

Wang, Shizhong; Wu, Lingli; Gao, Jie; He, Qiong; Liu, Meilin

The transference numbers for oxygen ion (t O) in several LaGaO 3-based materials are determined from oxygen concentration cells using the materials as the electrolyte, including La 0.8Sr 0.2Ga 0.8Mg 0.2O 3- δ (LSGM8282), La 0.8Sr 0.2Ga 0.8Mg 0.15Co 0.05O 3- δ (LSGMC5) and La 0.8Sr 0.2Ga 0.8Mg 0.115Co 0.085O 3- δ (LSGMC8.5). Analysis indicates that the accuracy in determination of oxygen ion transference number depends on the electrode polarization resistances of the concentration cell as well as the transport properties of the materials studied. For example, the ratio of open cell voltage to Nernst potential is a good approximation to the ionic transference number for LSGM8282. However, this approximation is no longer adequate for LSGMC5 and LSGMC8.5; the effect of electrode polarization resistances must be taken into consideration in estimation of the ionic transference numbers. In particular, the ionic transference number for LSGMC5 is as high as 0.99, suggesting that it is a promising electrolyte material for low-temperature solid-state electrochemical applications.

Polarization measurement for internal polarized gaseous targets

International Nuclear Information System (INIS)

Ye Zhenyu; Ye Yunxiu; Lv Haijiang; Mao Yajun

2004-01-01

The authors present an introduction to internal polarized gaseous targets, polarization method, polarization measurement method and procedure. To get the total nuclear polarization of hydrogen atoms (including the polarization of the recombined hydrogen molecules) in the target cell, authors have measured the parameters relating to atomic polarization and polarized hydrogen atoms and molecules. The total polarization of the target during our measurement is P T =0.853 ± 0.036. (authors)

Diurnal and seasonal occurrence of polar patches

Directory of Open Access Journals (Sweden)

A. S. Rodger

1996-05-01

Full Text Available Analysis of the diurnal and seasonal variation of polar patches, as identified in two years of HF-radar data from Halley, Antarctica during a period near sunspot maximum, shows that there is a broad maximum in occurrence centred about magnetic noon, not local noon. There are minima in occurrence near midsummer and midwinter, with maxima in occurrence between equinox and winter. There are no significant correlations between the occurrence of polar patches and the corresponding hourly averages of the solar wind and IMF parameters, except that patches usually occur when the interplanetary magnetic field has a southward component. The results can be understood in terms of UT and seasonal differences in the plasma concentration being convected from the dayside ionosphere into the polar cap. In summer and winter the electron concentrations in the polar cap are high and low, respectively, but relatively unstructured. About equinox, a tongue of enhanced ionisation is convected into the polar cap; this tongue is then structured by the effects of the interplanetary magnetic field, but these Halley data cannot be used to separate the various competing mechanisms for patch formation. The observed diurnal and seasonal variation in the occurrence of polar patches are largely consistent with predictions of Sojka et al. (1994 when their results are translated into the southern hemisphere. However, the ionospheric effects of flux transfer events are still considered essential in their formation, a feature not yet included in the Sojka et al. model.

The new polarized neutron reflectometer in Juelich

International Nuclear Information System (INIS)

Ruecker, U.; Alefeld, B.; Bergs, W.; Kentzinger, E.; Brueckel, T.

1999-01-01

On the basis of the HADAS spectrometer in the guide hall of the Juelich research reactor FRJ-2 a polarized neutron reflectometer is build with a 2D-position sensitive detector system. The new spectrometer is optimized for reflectivity and diffuse magnetic scattering measurements with small incident angles on thin magnetic films with thicknesses in the nm range. The polarization analyzer covers the whole detector area, so that a range of 2.5 deg in the scattering angle can be measured simultaneously. The analyzer consists of a stack of supermirrors tilted against the scattering plane. In this reflection geometry, the momentum transfer resolution of the instrument is not reduced, but the sample height is limited to 17 mm. For the monochromator, polarizer and collimation different setups have been compared on the basis of Monte-Carlo calculations: a focusing elliptical supermirror monochromator, a cylindrical mirror, a focusing pyrolytic graphite double monochromator and a double monochromator with bent perfect Si crystals. (author)

Recent progress on HYSPEC, and its polarization analysis capabilities

Directory of Open Access Journals (Sweden)

Winn Barry

2015-01-01

Full Text Available HYSPEC is a high-intensity, direct-geometry time-of-flight spectrometer at the Spallation Neutron Source, optimized for measurement of excitations in small single-crystal specimens with optional polarization analysis capabilities. The incident neutron beam is monochromated using a Fermi chopper with short, straight blades, and is then vertically focused by Bragg scattering onto the sample position by either a highly oriented pyrolitic graphite (unpolarized or a Heusler (polarized crystal array. Neutrons are detected by a bank of 3He tubes that can be positioned over a wide range of scattering angles about the sample axis. HYSPEC entered the user program in February 2013 for unpolarized experiments, and is already experiencing a vibrant research program. Polarization analysis will be accomplished by using the Heusler crystal array to polarize the incident beam, and either a 3He spin filter or a supermirror wide-angle polarization analyser to analyse the scattered beam. The 3He spin filter employs the spin-exchange optical pumping technique. A 60∘ wide angle 3He cell that matches the detector coverage will be used for polarization analysis. The polarized gas in the post-sample wide angle cell is designed to be periodically and automatically refreshed with an adjustable pressure of polarized gas, optically pumped in a separate cell and then transferred to the wide angle cell. The supermirror analyser has 960 supermirror polarizers distributed over 60∘, and has been characterized at the Swiss Spallation Neutron Source. The current status of the instrument and the development of its polarization analysis capabilities are presented.

Theory of radiative transfer in a strong magnetic field

Energy Technology Data Exchange (ETDEWEB)

Kanno, S [Ibaraki Univ., Mito (Japan). Dept. of Physics

1975-07-01

A theory is presented of the radiative transfer in a magnetized plasma with the opacity determined by the Thomson scattering. The Thomson cross section in the magnetic field is highly anisotropic and polarization-dependent. In order to cope with this situation, it is found useful to deal directly with the scattering amplitude (2x2 matrix in the polarization vector space) rather than the intensity. In this way it is possible to take into account the coherent superposition of the forward multiple-scattering amplitudes as a photon propagates. The equation of transfer is established accordingly and approximate solutions are found in the limits of small and large optical thickness. The latter solution is used to find the intensity and the polarization of thermal X-rays from a magnetic dipole star. The concept of mean free path is discussed and also it is shown that the Faraday rotation naturally comes about as a result of the multiple forward scattering.

Influence of aerosols, clouds, and sunglint on polarization spectra of Earthshine

Science.gov (United States)

Emde, Claudia; Buras-Schnell, Robert; Sterzik, Michael; Bagnulo, Stefano

2017-08-01

Context. Ground-based observations of the Earthshine, I.e., the light scattered by Earth to the Moon, and then reflected back to Earth, simulate space observations of our planet and represent a powerful benchmark for the studies of Earth-like planets. Earthshine spectra are strongly linearly polarized, owing to scattering by molecules and small particles in the atmosphere of the Earth and surface reflection, and may allow us to measure global atmospheric and surface properties of planet Earth. Aims: We aim to interpret already published spectropolarimetric observations of the Earthshine by comparing them with new radiative transfer model simulations including a fully realistic three-dimensional (3D) surface-atmosphere model for planet Earth. Methods: We used the highly advanced Monte Carlo radiative transfer model MYSTIC to simulate polarized radiative transfer in the atmosphere of the Earth without approximations regarding the geometry, taking into account the polarization from surface reflection and multiple scattering by molecules, aerosol particles, cloud droplets, and ice crystals. Results: We have shown that Earth spectropolarimetry is highly sensitive to all these input parameters, and we have presented simulations of a fully realistic Earth atmosphere-surface model including 3D cloud fields and two-dimensional (2D) surface property maps. Our modeling results show that scattering in high ice water clouds and reflection from the ocean surface are crucial to explain the continuum polarization at longer wavelengths as has been reported in Earthshine observations taken at the Very Large Telescope in 2011 (3.8% and 6.6% at 800 nm, depending on which part of Earth was visible from the Moon at the time of the observations). We found that the relatively high degree of polarization of 6.6% can be attributed to light reflected by the ocean surface in the sunglint region. High ice-water clouds reduce the amount of absorption in the O2A band and thus explain the weak O2

Plasmonic non-concentric nanorings array as an unidirectional nano-optical conveyor belt actuated by polarization rotation.

Science.gov (United States)

Jiang, Min; Wang, Guanghui; Jiao, Wenxiang; Ying, Zhoufeng; Zou, Ningmu; Ho, Ho-Pui; Sun, Tianyu; Zhang, Xuping

2017-01-15

We report a nano-optical conveyor belt containing an array of gold plasmonic non-concentric nanorings (PNNRs) for the realization of trapping and unidirectional transportation of nanoparticles through rotating the polarization of an excitation beam. The location of hot spots within an asymmetric plasmonic nanostructure is polarization dependent, thus making it possible to manipulate a trapped target by rotating the incident polarization state. In the case of PNNR, the two poles have highly unbalanced trap potential. This greatly enhances the chance of transferring trapped particles between adjacent PNNRs in a given direction through rotating the polarization. As confirmed by three-dimensional finite-difference time-domain analysis, an array of PNNRs forms an unidirectional nano-optical conveyor belt, which delivers target nanoparticles or biomolecules over a long distance with nanometer accuracy. With the capacity to trap and to transfer, our design offers a versatile scheme for conducting mechanical sample manipulation in many on-chip optofluidic applications.

Spin dependent fragmentation functions for heavy flavor baryons and single heavy hyperon polarization

CERN Document Server

Goldstein, G R

2001-01-01

Spin dependent fragmentation functions for heavy flavor quarks to fragment into heavy baryons are calculated in a quark-diquark model. The production of intermediate spin 1/2 and 3/2 excited states is explicity included. $\\Lambda_b$ , $\\Lambda_c$ and $\\Xi_c$ production rate and polarization at LEP energies are calculated and, where possible, compared with experiment. A different approach, also relying on a heavy quark-diquark model, is proposed for the small momentum transfer inclusive production of polarized heavy flavor hyperons. The predicted $\\Lambda_c$ polarization is roughly in agreement with experiment.

Estimation of land-atmosphere energy transfer over the Tibetan Plateau by a combination use of geostationary and polar-orbiting satellite data

Science.gov (United States)

Zhong, L.; Ma, Y.

2017-12-01

Land-atmosphere energy transfer is of great importance in land-atmosphere interactions and atmospheric boundary layer processes over the Tibetan Plateau (TP). The energy fluxes have high temporal variability, especially in their diurnal cycle, which cannot be acquired by polar-orbiting satellites alone because of their low temporal resolution. Therefore, it's of great practical significance to retrieve land surface heat fluxes by a combination use of geostationary and polar orbiting satellites. In this study, a time series of the hourly LST was estimated from thermal infrared data acquired by the Chinese geostationary satellite FengYun 2C (FY-2C) over the TP. The split window algorithm (SWA) was optimized using a regression method based on the observations from the Enhanced Observing Period (CEOP) of the Asia-Australia Monsoon Project (CAMP) on the Tibetan Plateau (CAMP/Tibet) and Tibetan observation and research platform (TORP), the land surface emissivity (LSE) from the Moderate Resolution Imaging Spectroradiometer (MODIS), and the water vapor content from the National Centers for Environmental Prediction (NCEP) Climate Forecast System Reanalysis (CFSR) project. The 10-day composite hourly LST data were generated via the maximum value composite (MVC) method to reduce the cloud effects. The derived LST was validated by the field observations of CAMP/Tibet and TORP. The results show that the retrieved LST and in situ data have a very good correlation (with root mean square error (RMSE), mean bias (MB), mean absolute error (MAE) and correlation coefficient (R) values of 1.99 K, 0.83 K, 1.71 K, and 0.991, respectively). Together with other characteristic parameters derived from polar-orbiting satellites and meteorological forcing data, the energy balance budgets have been retrieved finally. The validation results showed there was a good consistency between estimation results and in-situ measurements over the TP, which prove the robustness of the proposed estimation

Polarization observables in hard rescattering mechanism of deuteron photodisintegration

Energy Technology Data Exchange (ETDEWEB)

Sargsian, Misak M

2004-05-06

Polarization properties of high energy photodisintegration of the deuteron are studied within the framework of the hard rescattering mechanism (HRM). In HRM, a quark of one nucleon knocked-out by the incoming photon rescatters with a quark of the other nucleon leading to the production of two nucleons with high relative momentum. Summation of all relevant quark rescattering amplitudes allows us to express the scattering amplitude of the reaction through the convolution of a hard photon-quark interaction vertex, the large angle p-n scattering amplitude and the low momentum deuteron wave function. Within HRM, it is demonstrated that the polarization observables in hard photodisintegration of the deuteron can be expressed through the five helicity amplitudes of NN scattering at high momentum transfer. At 90 deg. CM scattering HRM predicts the dominance of the isovector channel of hard pn rescattering, and it explains the observed smallness of induced, P{sub y} and transfered, C{sub x} polarizations without invoking the argument of helicity conservation. Namely, HRM predicts that P{sub y} and C{sub x} are proportional to the phi{sub 5} helicity amplitude which vanishes at {theta}{sub cm}=90 deg. due to symmetry reasons. HRM predicts also a nonzero value for C{sub z} in the helicity-conserving regime and a positive {sigma} asymmetry which is related to the dominance of the isovector channel in the hard reinteraction. We extend our calculations to the region where large polarization effects are observed in pp scattering as well as give predictions for angular dependences.

Proton transfer dynamics in a polar nanodroplet: ESIPT of 4'-n,n-dimethylamino-3-hydroxyflavone in AOT/alkane/water reverse micelles

Energy Technology Data Exchange (ETDEWEB)

Ghosh, Deborin [Department of Chemistry, University College of Science & Technology, University of Calcutta, 92, A.P.C. Road, Kolkata 700 009 (India); Batuta, Shaikh; Begum, Naznin Ara [Bio-Organic Chemistry Lab, Department of Chemistry, Visva-Bharati University, Santiniketan 731 235 (India); Mandal, Debabrata, E-mail: dmandal.chemistry@gmail.com [Department of Chemistry, University College of Science & Technology, University of Calcutta, 92, A.P.C. Road, Kolkata 700 009 (India)

2017-04-15

The excited state intramolecular proton transfer (ESIPT) of the well-known fluorophore 4'-N,N-Dimethylamino-3-hydroxyflavone (DMA3HF) was studied in AOT/n-heptane/water reverse micelle solutions. For DMA3HF molecules located inside the AOT encapsulated polar nanodroplets, ESIPT from excited enol (E*) to tautomer (T*) forms was markedly inhibited, yielding time-constants of ≥100 ps, and followed the same trend as solvent relaxation when the ratio W= [H{sub 2}O]/[AOT] was varied. At W=0, the DMA3HF molecules were attached to the ionic AOT headgroups via strong intermolecular H-bonding, which hindered ESIPT. Addition of water changes the situation radically: water molecules form stronger H-bonds with AOT headgroups, displacing the DMA3HF, which are instead engaged in intermolecular H-bonded complexes of the type [DMA3HF···water]. ESIPT of these complex-bound fluorophores involves substantial rearrangement of H-bonding, and is coupled to solvation dynamics. With increasing W-value, solvation becomes faster, and so does ESIPT, reducing the yield of E* species. At the same time, the local environment within the nanodroplets become more more polar with gradual accumulation of water, which causes a monotonic red-shift of the E* emission peak.

How It's Made - Polarized Proton Beam (444th Brookhaven Lecture)

International Nuclear Information System (INIS)

Zelenski, Anatoli

2008-01-01

Experiments with polarized beams at RHIC will provide fundamental tests of QCD, and the electro-weak interaction reveal the spin structure of the proton. Polarization asymmetries and parity violation are the strong signatures for identification of the fundamental processes, which are otherwise inaccessible. Such experiments require the maximum available luminosity and therefore polarization must be obtained as an extra beam quality without sacrificing intensity. There are proposals to polarize the high-energy proton beam in the storage rings by the Stern-Gerlach effect or spin-filter techniques. But so far, the only practically available option is acceleration of the polarized beam produced in the source and taking care of polarization survival during acceleration and storage. Two major innovations -- the 'Siberian Snake' technique for polarization preservation during acceleration and high current polarized proton sources make spin physics with the high-energy polarized beams feasible. The RHIC is the first high-energy collider, where the 'Siberian Snake' technique allowed of polarized proton beam acceleration up-to 250 GeV energy. The RHIC unique Optically Pumped Polarized Ion Source produces sufficient polarized beam intensity for complete saturation of the RHIC acceptance. This polarization technique is based on spin-transfer collisions between a proton or atomic hydrogen beam of a few keV beam energy and optically pumped alkali metal vapors. From the first proposal and feasibility studies to the operational source this development can be considered as example of successful unification of individual scientists ingenuity, international collaboration and modern technology application for creation of a new polarization technique, which allowed of two-to-three order of magnitude polarized beam intensity increase sufficient for loading the RHIC to its full capacity for polarization studies.

7Li breakup polarization potential at near barrier energies

International Nuclear Information System (INIS)

Lubian, J. . E-mail lubian@if.uff.br; Correa, T.; Paes, B.; Figueira, J.M.; Abriola, D.; Fernandez Niello, J.O.; Arazi, A.; Capurro, O.A.; de Barbara, E.; Marti, G.V.; Martinez Heinmann, D.; Negri, A.E.; Pacheco, A.J.; Padron, I.; Gomes, P.R.S.

2007-01-01

Inelastic and one neutron transfer cross sections at energies around the Coulomb barrier were used to derive dynamic polarization potential (DPP) for the 7 Li + 27 Al system. The DPP due to breakup, obtained in a simple way, indicates that its real part is repulsive at near barrier energies

Observation of strongly forbidden solid effect dynamic nuclear polarization transitions via electron-electron double resonance detected NMR

Energy Technology Data Exchange (ETDEWEB)

Smith, Albert A.; Corzilius, Björn; Haze, Olesya; Swager, Timothy M.; Griffin, Robert G., E-mail: rgg@mit.edu [Department of Chemistry and Francis Bitter Magnet Laboratory, Massachusetts Institute of Technology, Cambridge, Massachusetts 02139 (United States)

2013-12-07

We present electron paramagnetic resonance experiments for which solid effect dynamic nuclear polarization transitions were observed indirectly via polarization loss on the electron. This use of indirect observation allows characterization of the dynamic nuclear polarization (DNP) process close to the electron. Frequency profiles of the electron-detected solid effect obtained using trityl radical showed intense saturation of the electron at the usual solid effect condition, which involves a single electron and nucleus. However, higher order solid effect transitions involving two, three, or four nuclei were also observed with surprising intensity, although these transitions did not lead to bulk nuclear polarization—suggesting that higher order transitions are important primarily in the transfer of polarization to nuclei nearby the electron. Similar results were obtained for the SA-BDPA radical where strong electron-nuclear couplings produced splittings in the spectrum of the indirectly observed solid effect conditions. Observation of high order solid effect transitions supports recent studies of the solid effect, and suggests that a multi-spin solid effect mechanism may play a major role in polarization transfer via DNP.

Atmospheres and spectra of strongly magnetized neutron stars - II. The effect of vacuum polarization

Science.gov (United States)

Ho, Wynn C. G.; Lai, Dong

2003-01-01

We study the effect of vacuum polarization on the atmosphere structure and radiation spectra of neutron stars with surface magnetic fields B= 1014-1015 G, as appropriate for magnetars. Vacuum polarization modifies the dielectric property of the medium and gives rise to a resonance feature in the opacity; this feature is narrow and occurs at a photon energy that depends on the plasma density. Vacuum polarization can also induce resonant conversion of photon modes via a mechanism analogous to the Mikheyev-Smirnov-Wolfenstein (MSW) mechanism for neutrino oscillation. We construct atmosphere models in radiative equilibrium with an effective temperature of a few ×106 K by solving the full radiative transfer equations for both polarization modes in a fully ionized hydrogen plasma. We discuss the subtleties in treating the vacuum polarization effects in the atmosphere models and present approximate solutions to the radiative transfer problem which bracket the true answer. We show from both analytic considerations and numerical calculations that vacuum polarization produces a broad depression in the X-ray flux at high energies (a few keV <~E<~ a few tens of keV) as compared to models without vacuum polarization; this arises from the density dependence of the vacuum resonance feature and the large density gradient present in the atmosphere. Thus the vacuum polarization effect softens the high-energy tail of the thermal spectrum, although the atmospheric emission is still harder than the blackbody spectrum because of the non-grey opacities. We also show that the depression of continuum flux strongly suppresses the equivalent width of the ion cyclotron line and therefore makes the line more difficult to observe.

Exploring the Effects of Cloud Vertical Structure on Cloud Microphysical Retrievals based on Polarized Reflectances

Science.gov (United States)

Miller, D. J.; Zhang, Z.; Platnick, S. E.; Ackerman, A. S.; Cornet, C.; Baum, B. A.

2013-12-01

A polarized cloud reflectance simulator was developed by coupling an LES cloud model with a polarized radiative transfer model to assess the capabilities of polarimetric cloud retrievals. With future remote sensing campaigns like NASA's Aerosols/Clouds/Ecosystems (ACE) planning to feature advanced polarimetric instruments it is important for the cloud remote sensing community to understand the retrievable information available and the related systematic/methodical limitations. The cloud retrieval simulator we have developed allows us to probe these important questions in a realistically relevant test bed. Our simulator utilizes a polarized adding-doubling radiative transfer model and an LES cloud field from a DHARMA simulation (Ackerman et al. 2004) with cloud properties based on the stratocumulus clouds observed during the DYCOMS-II field campaign. In this study we will focus on how the vertical structure of cloud microphysics can influence polarized cloud effective radius retrievals. Numerous previous studies have explored how retrievals based on total reflectance are affected by cloud vertical structure (Platnick 2000, Chang and Li 2002) but no such studies about the effects of vertical structure on polarized retrievals exist. Unlike the total cloud reflectance, which is predominantly multiply scattered light, the polarized reflectance is primarily the result of singly scattered photons. Thus the polarized reflectance is sensitive to only the uppermost region of the cloud (tau~influencer on the microphysical development of cloud droplets, can be potentially studied with polarimetric retrievals.

Broadband polarized emission from P(NDI2OD-T2) polymer.

Science.gov (United States)

Ulrich, Steve; Sutch, Tabitha; Szulczewski, Greg; Schweizer, Matthias; Barbosa, Newton; Araujo, Paulo

2018-05-18

We investigate the P(NDI2OD-T2) photophysical properties via absorbance and fluorescence spectroscopy, in association with the experimental approach baptized Stokes Spectroscopy, which provides valuable material information through the acquisition and analysis of the fluorescence polarization degree. By changing solvents and using different samples such as solutions, thick, and thin films, it is possible to control the polarization degree spectrum associated to the fluorescence emitted by the polymer's isolated chains and aggregates. We show that the polarization degree could become a powerful tool to obtain information related to the samples morphology, which is connected to their microscopic structure. Moreover, the polarization degree spectra suggest that depolarization effects linked to energy and charge transfer mechanisms are likely taking place. Our findings indicate that P(NDI2OD-T2) polymers are excellent candidates for the advancement of organic technologies that rely on the emission and detection of polarized lights. © 2018 IOP Publishing Ltd.

Polarized tagged photons

International Nuclear Information System (INIS)

Maximon, L.C.; Ganz, Eric; Aniel, Thierry; Miniac, Arlette de.

1982-03-01

We consider in detail the differential cross section for polarized bremsstrahlung for angles and energies in the range of interest for a tagging system and derive a high energy, small angle approximation for this cross section. We use these approximations to determine the maxima and minima of the cross sections for these two polarization states, dσperpendicular and dσparallel, and to evaluate these cross sections at the extrema. It is shown that both dσperpendicular and dσparallel have a very sharp dip in the region of small momentum transfers. However, their behavior in the region of the dip, as a function of the azimuthal angle phi, is quite different over most of the photon spectrum. The cross section dσperpendicular behaves similarly to the cross section for unpolarized photons in that as phi increases, the sharp dip vanishes, the minimum fuses with the second maximum, and the cross section then has only a single maximum. In contrast, the sharp dip in the cross section dσparallel remains as phi increases. Coulomb corrections to the Born approximation are considered, and do not fill in these dips

Optically enhanced nuclear cross polarization in acridine-doped fluorene

Energy Technology Data Exchange (ETDEWEB)

Oshiro, C.M.

1982-06-01

The objective of this work has been to create large polarizations of the dilute /sup 13/C nuclei in the solid state. The idea was to create /sup 1/H polarizations larger than Boltzmann and to use the proton enhanced nuclear induction spectroscopy cross polarization technique to then transfer this large polarization to the /sup 13/C spin system. Optical Nuclear Polarization (ONP) of acridine-doped fluorene single crystals was studied. In addition, ONP of powdered samples of the acridine-doped fluorene was studied. In general, many compounds do not crystallize easily or do not form large crystals suitable for NMR experiments. Powdered, amorphous and randomly dispersed samples are generally far more readily available than single crystals. One objective of this work has been to (first) create large /sup 1/H polarizations. Although large optical proton polarizations in single crystals have been reported previously, optically generated polarizations in powdered samples have not been reported. For these reasons, ONP studies of powdered samples of the acridine-doped fluorene were also undertaken. Using ONP in combination with the proton enhanced nuclear induction spectroscopy experiment, large /sup 13/C polarizations have been created in fluorene single crystals. These large /sup 13/C polarizations have permitted the determination of the seven incongruent chemical shielding tensors of the fluorene molecule. Part 2 of this thesis describes the proton enhanced nuclear induction spectroscopy experiment. Part 3 describes the ONP experiment. Part 4 is a description of the experimental set-up. Part 5 describes the data analysis for the determination of the chemical shielding tensors. Part 6 presents the results of the ONP experiments performed in this work and the chemical shielding tensors determined.

Optically enhanced nuclear cross polarization in acridine-doped fluorene

International Nuclear Information System (INIS)

Oshiro, C.M.

1982-06-01

The objective of this work has been to create large polarizations of the dilute 13 C nuclei in the solid state. The idea was to create 1 H polarizations larger than Boltzmann and to use the proton enhanced nuclear induction spectroscopy cross polarization technique to then transfer this large polarization to the 13 C spin system. Optical Nuclear Polarization (ONP) of acridine-doped fluorene single crystals was studied. In addition, ONP of powdered samples of the acridine-doped fluorene was studied. In general, many compounds do not crystallize easily or do not form large crystals suitable for NMR experiments. Powdered, amorphous and randomly dispersed samples are generally far more readily available than single crystals. One objective of this work has been to (first) create large 1 H polarizations. Although large optical proton polarizations in single crystals have been reported previously, optically generated polarizations in powdered samples have not been reported. For these reasons, ONP studies of powdered samples of the acridine-doped fluorene were also undertaken. Using ONP in combination with the proton enhanced nuclear induction spectroscopy experiment, large 13 C polarizations have been created in fluorene single crystals. These large 13 C polarizations have permitted the determination of the seven incongruent chemical shielding tensors of the fluorene molecule. Part 2 of this thesis describes the proton enhanced nuclear induction spectroscopy experiment. Part 3 describes the ONP experiment. Part 4 is a description of the experimental set-up. Part 5 describes the data analysis for the determination of the chemical shielding tensors. Part 6 presents the results of the ONP experiments performed in this work and the chemical shielding tensors determined

Measurement of Polarization Observables in the Electro-Excitation of the Proton to its First Excited State

International Nuclear Information System (INIS)

Rikki Roche

2003-01-01

This thesis reports results from the Thomas Jefferson National Accelerator Facility (Jefferson Lab) Hall A experiment E91-011, which measured double-polarization observables in the pion electroproduction reaction from the proton. Specifically, the experiment measured the recoil proton polarization, polarized response functions, and cross section for the p(rvec e), e(prime) (rvec p) π o reaction at a center-of-mass energy centered at W = 1232 MeV--the peak of the Δ(1232) resonance--and at a four-momentum transfer squared of Q 2 = 1.0 GeV 2 /c 2 . Both the recoil proton polarization and polarized response function results will be presented in this thesis

Oxygen ion transference number of doped lanthanum gallate

Energy Technology Data Exchange (ETDEWEB)

Wang, Shizhong; Wu, Lingli; Gao, Jie; He, Qiong [Department of Chemistry, College of Chemistry and Chemical Engineering, Xiamen University, Xiamen, Fujian 361005 (China); Liu, Meilin [School of Materials Science and Engineering, Georgia Institute of Technology, Atlanta, GA 30332-0245 (United States)

2008-12-01

The transference numbers for oxygen ion (t{sub O}) in several LaGaO{sub 3}-based materials are determined from oxygen concentration cells using the materials as the electrolyte, including La{sub 0.8}Sr{sub 0.2}Ga{sub 0.8}Mg{sub 0.2}O{sub 3-{delta}} (LSGM8282), La{sub 0.8}Sr{sub 0.2}Ga{sub 0.8}Mg{sub 0.15}Co{sub 0.05}O{sub 3-{delta}} (LSGMC5) and La{sub 0.8}Sr{sub 0.2}Ga{sub 0.8}Mg{sub 0.115}Co{sub 0.085}O{sub 3-{delta}} (LSGMC8.5). Analysis indicates that the accuracy in determination of oxygen ion transference number depends on the electrode polarization resistances of the concentration cell as well as the transport properties of the materials studied. For example, the ratio of open cell voltage to Nernst potential is a good approximation to the ionic transference number for LSGM8282. However, this approximation is no longer adequate for LSGMC5 and LSGMC8.5; the effect of electrode polarization resistances must be taken into consideration in estimation of the ionic transference numbers. In particular, the ionic transference number for LSGMC5 is as high as 0.99, suggesting that it is a promising electrolyte material for low-temperature solid-state electrochemical applications. (author)

Polarized 3He Gas Circulating Technologies for Neutron Analyzers

Energy Technology Data Exchange (ETDEWEB)

Watt, David [Xemed LLC, Durham, NH (United States); Hersman, Bill [Xemed LLC, Durham, NH (United States)

2014-12-10

We describe the development of an integrated system for quasi-continuous operation of a large volume neutron analyzer. The system consists of a non-magnetic diaphragm compressor, a prototype large volume helium polarizer, a surrogate neutron analyzer, a non-depolarizing gas storage reservoir, a non-ferrous valve manifold for handling gas distribution, a custom rubidium-vapor gas return purifier, and wire-wound transfer lines, all of which are immersed in a two-meter external magnetic field. Over the Phase II period we focused on three major tasks required for the successful deployment of these types of systems: 1) design and implementation of gas handling hardware, 2) automation for long-term operation, and 3) improvements in polarizer performance, specifically fabrication of aluminosilicate optical pumping cells. In this report we describe the design, implementation, and testing of the gas handling hardware. We describe improved polarizer performance resulting from improved cell materials and fabrication methods. These improvements yielded valved 8.5 liter cells with relaxation times greater than 12 hours. Pumping this cell with 1500W laser power with 1.25nm linewidth yielded peak polarizations of 60%, measured both inside and outside the polarizer. Fully narrowing this laser to 0.25nm, demonstrated separately on one stack of the four, would have allowed 70% polarization with this cell. We demonstrated the removal of 5 liters of polarized helium from the polarizer with no measured loss of polarization. We circulated the gas through a titanium-clad compressor with polarization loss below 3% per pass. We also prepared for the next phase of development by refining the design of the polarizer so that it can be engineer-certified for pressurized operation. The performance of our system far exceeds comparable efforts elsewhere.

Photo-Induced Electron Spin Polarization in a Narrow Band Gap Semiconductor Nanostructure

International Nuclear Information System (INIS)

Peter, A. John; Lee, Chang Woo

2012-01-01

Photo-induced spin dependent electron transmission through a narrow gap InSb/InGa x Sb 1−x semiconductor symmetric well is theoretically studied using transfer matrix formulism. The transparency of electron transmission is calculated as a function of electron energy for different concentrations of gallium. Enhanced spin-polarized photon assisted resonant tunnelling in the heterostructure due to Dresselhaus and Rashba spin-orbit coupling induced splitting of the resonant level and compressed spin-polarization are observed. Our results show that Dresselhaus spin-orbit coupling is dominant for the photon effect and the computed polarization efficiency increases with the photon effect and the gallium concentration

Theoretical aspects of electron transfer reactions of complex molecules

DEFF Research Database (Denmark)

Kuznetsov, A. M.; Ulstrup, Jens

2001-01-01

Features of electron transfer involving complex molecules are discussed. This notion presently refers to molecular reactants where charge transfer is accompanied by large molecular reorganization, and commonly used displaced harmonic oscillator models do not apply. It is shown that comprehensive...... theory of charge transfer in polar media offers convenient tools for the treatment of experimental data for such systems, with due account of large-amplitude strongly anharmonic intramolecular reorganization. Equations for the activation barrier and free energy relationships are provided, incorporating...

Effect of solvent polarity and temperature on the spectral and thermodynamic properties of exciplexes of 1-cyanonaphthalene with hexamethylbenzene in organic solvents

International Nuclear Information System (INIS)

Asim, Sadia; Mansha, Asim; Grampp, Günter; Landgraf, Stephan; Zahid, Muhammad; Bhatti, Ijaz Ahmad

2014-01-01

Study of the effect of solvent polarity and temperature is done on the exciplex emission spectra of 1-cyanonaphthalene with hexamethylbenzene. Exciplex system is studied in the range of partially polar solvents and in solvent mixture of propyl acetate and butyronitrile. The unique feature of this solvent mixture is that only the solvent polarity changes (6.0≤ε s ≤24.7) with the change in the mole fraction of solvents whereas the solvent viscosity and refractive index remains unaffected. Thermodynamic properties are calculated according to the models developed by Weller and Kuzmin. Fluorescence lifetimes for both the fluorophore as well as the exciplex are evaluated in all used solvents. Exciplex energetics as a function of solvent polarity and temperature are also discussed. Kuzmin model of self-consistent polarization is used for the explanation of the exciplex emission spectra. The effects of solvent polarity and temperature on energy of zero–zero transitions (hv 0 / ), Huang–Rhys factor (S), Gauss broadening of vibronic level (σ) and the dominant high-frequency vibration (hν ν ) are investigated. The strong dependence of exciplex stability and energetics upon the solvent polarity and temperature are observed. Full charge transfer exciplexes were observed in solvents of all polarities and stronger exciplex with large emission intensities were found in solvents of low polarities but with the increase in solvent polarity the exciplex becomes weak and they dissociate fastly into radical ion pairs. The kinetic model of Kuzmin was observed to reduce into the Weller kinetic model for this exciplex system with ∆G ET = −0.22 eV and the spectral shift, h∆ν>0.2 eV. - Highlights: • Exciplex formed as a result of mixing of charge transfer and locally excited states. • Effect of solvents polarity and temperature on the exciplex stability and thermodynamics. • Solvent polarity will decide the formation of contact radical ion pair or solvent separated

np Elastic-scattering experiments with polarized neutron beams

International Nuclear Information System (INIS)

Chalmers, J.S.; Ditzler, W.R.; Hill, D.

1985-01-01

Measurements of the spin transfer parameters, K/sub NN/ and K/sub LL/, at 500, 650, and 800 MeV are presented for the reaction p-vector d → n-vector pp at 0 0 . The data are useful input to the NN data base and indicate that the quasi-free charge exchange (CEX) reaction is a useful mechanism for producing neutrons with at least 40% polarization at energies as low as 500 MeV. Measurements of np elastic scattering observables C/sub LL/ and C/sub SL/ covering 35 0 to 172 0 are performed using a polarized neutron beam at 500, 650, and 800 MeV. Preliminary results are presented. 3 refs., 6 figs

Polarization spectrum of supernova 1987A interpreted in terms of shape asymmetry

Energy Technology Data Exchange (ETDEWEB)

Jeffery, D J

1987-10-01

Polarimetry carried out on the type II supernova 1987A on 6 and 7 March 1987 showed variation in polarization across line profiles. This polarization structure is interpreted as arising from an asymmetric, homologously expanding, scattering atmosphere surrounding an asymmetric continuum-producing photosphere. Resonant scattering of radiation by ions in the atmosphere produces the line structure in the flux spectrum and polarizes the emergent radiation. The asymmetric shape of the atmosphere causes a non-zero net polarization. Sobolev-method radiative transfer calculations with axisymmetric oblate ellipsoidal models have been carried out to fit the observed data. The models are parameterized by the ratio of the symmetry axis to the perpendicular axis, c/a. The fits to the 1987A data indicate that (c/a) is approx. 0.6-0.8.

Semileptonic weak and electromagnetic interactions in nuclei: recoil polarization in muon capture

International Nuclear Information System (INIS)

Rosenfelder, R.

1979-01-01

An analysis of the polarization of the recoiling nucleus following the capture of polarized muons by nuclei is performed. New general expressions for arbitrary nuclear spin are obtained in terms of the same reduced matrix elements which govern inelastic electron scattering and β-decay. As an application the A = 12 system is considered and uncertainties in the nuclear structure are studied by using different sets of one-body density matrices. With the canonical values of the weak form factors (i.e. absence of second-class currents) a fairly good agreement with the experimental data is achieved including the inelastic form factor at high momentum transfers and the recently measured average 12 B polarization. Implications of the new corrected value of the average polarization on weak form factors and nuclear structure are discussed. (Auth.)

Tantalum surface oxidation: Bond relaxation, energy entrapment, and electron polarization

Energy Technology Data Exchange (ETDEWEB)

Guo, Yongling [Key Laboratory of Low-Dimensional Materials and Application Technologies (Ministry of Education), Hunan Provincial Key Laboratory of Thin Film Materials and Devices, Faculty of Materials Science and Engineering, Xiangtan University, Hunan 411105 (China); Bo, Maolin [Yangtze Normal University, College of Mechanical and Electrical Engineering, Chongqing 408100 (China); Wang, Yan [School of Information and Electronic Engineering, Hunan University of Science and Technology, Hunan 411201 (China); Liu, Yonghui [Key Laboratory of Low-Dimensional Materials and Application Technologies (Ministry of Education), Hunan Provincial Key Laboratory of Thin Film Materials and Devices, Faculty of Materials Science and Engineering, Xiangtan University, Hunan 411105 (China); Sun, Chang Q. [NOVITAS, School of Electrical and Electronic Engineering, Nanyang Technological University, Singapore 639798 (Singapore); Huang, Yongli, E-mail: huangyongli@xtu.edu.cn [Key Laboratory of Low-Dimensional Materials and Application Technologies (Ministry of Education), Hunan Provincial Key Laboratory of Thin Film Materials and Devices, Faculty of Materials Science and Engineering, Xiangtan University, Hunan 411105 (China)

2017-02-28

Graphical abstract: The bond, electron and energy relaxation result in core level energy shift, local densification, quantum entrapment and electron polarization of bonding electrons. - Highlights: • Increasing the oxygen coverage lowers the adsorption energy associated with lattice reconstruction. • Electrons transfer from Ta surface atoms to sp-hydrated oxygen, creating dipole moment that decreases the work function. • Oxygen chemisorption modified valence density-of-state (DOS) for Ta with four excessive DOS features: O−Ta bonding, O{sup 2−} lone pairs, Ta+ electron holes, and the lone-pair polarized Ta dipoles. • The bond, electron and energy relaxation between surface undercoordinated atoms are responsible for core level energy shift, local densification, quantum entrapment and electron polarization of bonding electrons. - Abstract: A combination of photoelectron spectrometric analysis and density functional theory calculations has enabled reconciliation of the bond-energy-electron relaxation for the Ta(100, 110, 111) surfaces chemisorbed with oxygen at different coverages. Results show that increasing oxygen coverage lowers the adsorption energy associated with lattice reconstruction. Valence electrons transfer from Ta surface atoms to oxygen to create four excessive DOS features in terms of O−Ta bonding, lone pairs of oxygen, Ta{sup +} electron holes, and polarized Ta dipoles. Oxidation proceeds in the following dynamics: oxygen gets electrons from two neighboring Ta atoms left behind Ta{sup +}; the sp{sup 3}-orbital hybridization takes place with additional two electron lone pairs, the lone pairs polarize the other two Ta neighbors becoming dipoles. X-ray photoelectron spectral analysis results in the 4f binding energy of an isolated Ta atom and its shift upon bond formation and oxidation. Exercises provide not only a promising numerical approach for the quantitative information about the bond and electronic behavior but also consistent

Tantalum surface oxidation: Bond relaxation, energy entrapment, and electron polarization

International Nuclear Information System (INIS)

Guo, Yongling; Bo, Maolin; Wang, Yan; Liu, Yonghui; Sun, Chang Q.; Huang, Yongli

2017-01-01

Graphical abstract: The bond, electron and energy relaxation result in core level energy shift, local densification, quantum entrapment and electron polarization of bonding electrons. - Highlights: • Increasing the oxygen coverage lowers the adsorption energy associated with lattice reconstruction. • Electrons transfer from Ta surface atoms to sp-hydrated oxygen, creating dipole moment that decreases the work function. • Oxygen chemisorption modified valence density-of-state (DOS) for Ta with four excessive DOS features: O−Ta bonding, O"2"− lone pairs, Ta+ electron holes, and the lone-pair polarized Ta dipoles. • The bond, electron and energy relaxation between surface undercoordinated atoms are responsible for core level energy shift, local densification, quantum entrapment and electron polarization of bonding electrons. - Abstract: A combination of photoelectron spectrometric analysis and density functional theory calculations has enabled reconciliation of the bond-energy-electron relaxation for the Ta(100, 110, 111) surfaces chemisorbed with oxygen at different coverages. Results show that increasing oxygen coverage lowers the adsorption energy associated with lattice reconstruction. Valence electrons transfer from Ta surface atoms to oxygen to create four excessive DOS features in terms of O−Ta bonding, lone pairs of oxygen, Ta"+ electron holes, and polarized Ta dipoles. Oxidation proceeds in the following dynamics: oxygen gets electrons from two neighboring Ta atoms left behind Ta"+; the sp"3-orbital hybridization takes place with additional two electron lone pairs, the lone pairs polarize the other two Ta neighbors becoming dipoles. X-ray photoelectron spectral analysis results in the 4f binding energy of an isolated Ta atom and its shift upon bond formation and oxidation. Exercises provide not only a promising numerical approach for the quantitative information about the bond and electronic behavior but also consistent insight into the

Optically initialized robust valley-polarized holes in monolayer WSe2

KAUST Repository

Hsu, Wei-Ting

2015-11-25

A robust valley polarization is a key prerequisite for exploiting valley pseudospin to carry information in next-generation electronics and optoelectronics. Although monolayer transition metal dichalcogenides with inherent spin–valley coupling offer a unique platform to develop such valleytronic devices, the anticipated long-lived valley pseudospin has not been observed yet. Here we demonstrate that robust valley-polarized holes in monolayer WSe2 can be initialized by optical pumping. Using time-resolved Kerr rotation spectroscopy, we observe a long-lived valley polarization for positive trion with a lifetime approaching 1 ns at low temperatures, which is much longer than the trion recombination lifetime (~10–20 ps). The long-lived valley polarization arises from the transfer of valley pseudospin from photocarriers to resident holes in a specific valley. The optically initialized valley pseudospin of holes remains robust even at room temperature, which opens up the possibility to realize room-temperature valleytronics based on transition metal dichalcogenides.

Building Transferable Knowledge and Skills through an Interdisciplinary Polar Science Graduate Program

Science.gov (United States)

Culler, L. E.; Virginia, R. A.; Albert, M. R.; Ayres, M.

2015-12-01

Modern graduate education must extend beyond disciplinary content to prepare students for diverse careers in science. At Dartmouth, a graduate program in Polar Environmental Change uses interdisciplinary study of the polar regions as a core from which students develop skills and knowledge for tackling complex environmental issues that require cooperation across scientific disciplines and with educators, policy makers, and stakeholders. Two major NSF-funded initiatives have supported professional development for graduate students in this program, including an IGERT (Integrative Graduate Education and Research Traineeship) and leadership of JSEP's (Joint Science Education Project) Arctic Science Education Week in Greenland. We teach courses that emphasize the links between science and the human dimensions of environmental change; host training sessions in science communication; invite guest speakers who work in policy, academia, journalism, government research, etc.; lead an international field-based training that includes policy-focused meetings and a large outreach component; provide multiple opportunities for outreach and collaboration with local schools; and build outreach and education into graduate research programs where students instruct and mentor high school students. Students from diverse scientific disciplines (Ecology, Earth Science, and Engineering) participate in all of the above, which significantly strengthens their interdisciplinary view of polar science and ability to communicate across disciplines. In addition, graduate students have developed awareness, confidence, and the skills to pursue and obtain diverse careers. This is reflected in the fact that recent graduates have acquired permanent and post-doctoral positions in academic and government research, full-time teaching, and also in post-docs focused on outreach and science policy. Dartmouth's interdisciplinary approach to graduate education is producing tomorrow's leaders in science.

The impact of Faraday effects on polarized black hole images of Sagittarius A*.

Science.gov (United States)

Jiménez-Rosales, Alejandra; Dexter, Jason

2018-05-01

We study model images and polarization maps of Sagittarius A* at 230 GHz. We post-process GRMHD simulations and perform a fully relativistic radiative transfer calculation of the emitted synchrotron radiation to obtain polarized images for a range of mass accretion rates and electron temperatures. At low accretion rates, the polarization map traces the underlying toroidal magnetic field geometry. At high accretion rates, we find that Faraday rotation internal to the emission region can depolarize and scramble the map. We measure the net linear polarization fraction and find that high accretion rate "jet-disc" models are heavily depolarized and are therefore disfavoured. We show how Event Horizon Telescope measurements of the polarized "correlation length" over the image provide a model-independent upper limit on the strength of these Faraday effects, and constrain plasma properties like the electron temperature and magnetic field strength.

Measurements of Polarization Transfers in Real Compton Scattering by a proton target at JLAB. A new source of information on the 3D shape of the nucleon

Energy Technology Data Exchange (ETDEWEB)

Fanelli, Cristiano V. [Sapienza Univ. of Rome (Italy)

2015-03-01

In this thesis work, results of the analysis of the polarization transfers measured in real Compton scattering (RCS) by the Collaboration E07-002 at the Je fferson Lab Hall-C are presented. The data were collected at large scattering angle (theta_cm = 70deg) and with a polarized incident photon beam at an average energy of 3.8 GeV. Such a kind of experiments allows one to understand more deeply the reaction mechanism, that involves a real photon, by extracting both Compton form factors and Generalized Parton Distributions (GPDs) (also relevant for possibly shedding light on the total angular momentum of the nucleon). The obtained results for the longitudinal and transverse polarization transfers K_LL and K_LT, are of crucial importance, since they confirm unambiguously the disagreement between experimental data and pQCD prediction, as it was found in E99-114 experiment, and favor the Handbag mechanism. The E99-114 and E07-002 results can contribute to attract new interest on the great yield of the Compton scattering by a nucleon target, as demonstrated by the recent approval of an experimental proposal submitted to the Jefferson Lab PAC 42 for a Wide-angle Compton Scattering experiment, at 8 and 10 GeV Photon Energies. The new experiments approved to run with the updated 12 GeV electron beam at JLab, are characterized by much higher luminosities, and a new GEM tracker is under development to tackle the challenging backgrounds. Within this context, we present a new multistep tracking algorithm, based on (i) a Neural Network (NN) designed for a fast and efficient association of the hits measured by the GEM detector which allows the track identification, and (ii) the application of both a Kalman filter and Rauch-Tung-Striebel smoother to further improve the track reconstruction. The full procedure, i.e. NN and filtering, appears very promising, with high performances in terms of both association effciency and reconstruction accuracy, and these preliminary results will

Light scattering reviews 7 radiative transfer and optical properties of atmosphere and underlying surface

CERN Document Server

Kokhanovsky, Alexander A

2014-01-01

This book describes modern advances in radiative transfer and light scattering. Coverage includes fast radiative transfer techniques, use of polarization in remote sensing and recent developments in remote sensing of snow properties from space observations.

Polarization phenomena in quantum chromodynamics

Energy Technology Data Exchange (ETDEWEB)

Brodsky, S.J. [Stanford Univ., CA (United States)

1994-12-01

The author discusses a number of interrelated hadronic spin effects which test fundamental features of perturbative and nonperturbative QCD. For example, the anomalous magnetic moment of the proton and the axial coupling g{sub A} on the nucleon are shown to be related to each other for fixed proton radius, independent of the form of the underlying three-quark relativistic quark wavefunction. The renormalization scale and scheme ambiguities for the radiative corrections to the Bjorken sum rule for the polarized structure functions can be eliminated by using commensurate scale relations with other observables. Other examples include (a) new constraints on the shape and normalization of the polarized quark and gluon structure functions of the proton at large and small x{sub bj}; (b) consequences of the principle of hadron retention in high x{sub F} inclusive reactions; (c) applications of hadron helicity conservation to high momentum transfer exclusive reactions; and (d) the dependence of nuclear structure functions and shadowing on virtual photon polarization. The author also discusses the implications of a number of measurements which are in striking conflict with leading-twist perturbative QCD predictions, such as the extraordinarily large spin correlation A{sub NN} observed in large angle proton-proton scattering, the anomalously large {rho}{pi} branching ratio of the J/{psi}, and the rapidly changing polarization dependence of both J/{psi} and continuum lepton pair hadroproduction observed at large x{sub F}. The azimuthal angular dependence of the Drell-Yan process is shown to be highly sensitive to the projectile distribution amplitude, the fundamental valence light-cone wavefunction of the hadron.

Polarization phenomena in quantum chromodynamics

International Nuclear Information System (INIS)

Brodsky, S.J.

1994-03-01

The author discusses a number of interrelated hadronic spin effects which test fundamental features of perturbative and non-perturbative QCD. For example, the anomalous magnetic moment of the proton and the axial coupling g A on the nucleon are shown to be related to each other for fixed proton radius, independent of the form of the underlying three-quark relativistic quark wavefunction. The renormalization scale and scheme ambiguities for the radiative corrections to the Bjorken sum rule for the polarized structure functions can be eliminated by using commensurate scale relations with other observables. Other examples include (a) new constraints on the shape and normalization of the polarized quark and gluon structure functions of the proton at large and small x bj ; (b) consequences of the principle of hadron helicity retention in high x F inclusive reactions; (c) applications of hadron helicity conservation to high momentum transfer exclusive reactions; and (d) the dependence of nuclear structure functions and shadowing on virtual photon polarization. He also discusses the implications of a number of measurements which are in striking conflict with leading-twist perturbative QCD predictions, such as the extraordinarily large spin correlation A NN observed in large angle proton-proton scattering, the anomalously large ρπ branching ratio of the J/ψ, and the rapidly changing polarization dependence of both J/ψ and continuum lepton pair hadroproduction observed at large x F . The azimuthal angular dependence of the Drell-Yan process is shown to be highly sensitive to the projectile distribution amplitude, the fundamental valence light-cone wavefunction of the hadron

[Polarized light microscopy for evaluation of oocytes as a prognostic factor in the evolution of a cycle in assisted reproduction].

Science.gov (United States)

González-Ortega, C; Cancino-Villarreal, P; Alonzo-Torres, V E; Martínez-Robles, I; Pérez-Peña, E; Gutiérrez-Gutiérrez, A M

2016-04-01

Identification of the best embryos to transfer is a key element for success in assisted reproduction. In the last decade, several morphological criteria of oocytes and embryos were evaluated with regard to their potential for predicting embryo viability. The introduction of polarization light microscopy systems has allowed the visualization of the meiotic spindle and the different layers of the zona pellucida in human oocytes on the basis of birefringence in a non-destructive way. Conflicting results have been reported regarding the predictive value in ICSI cycles. To assess the predictive ability of meiotic spindle and zona pellucida of human oocytes to implant by polarized microscopy in ICSI cycles. Prospective and observational clinical study. 903 oocytes from 94 ICSI cycles were analyzed with polarized microscopy. Meiotic spindle visualization and zona pellucida birefringence values by polarized microscopy were correlated with ICSI cycles results. Meiotic spindle visualization and birefringence values of zona pellucida decreased in a direct basis with increasing age. In patients aged over the 35 years, the percentage of a visible spindle and mean zona pellucida birefringence was lower than in younger patients. Fertilization rate were higher in oocytes with visible meiotic spindle (81.3% vs. 64%; p vs. 39%; p=0.01). Fertilization rate was higher in oocytes with positive values of birefringence (77.5 % vs. 68.5% p=0.005) with similar embryo quality. Conception cycles showed oocytes with higher mean value of zona birefringence and visible spindle vs. no-conception cycles (pPolarized light microscopy improves oocyte selection, which significantly impacts in the development of embryos with greater implantation potential. The use of polarized light microscopy with sperm selection methods, blastocyst culture and deferred embryo transfers will contribute to transfer fewer embryos without diminishing rates of live birth and single embryo transfer will be more feasible.

Broadband working-waveband-tunable polarization converter based on anisotropic metasurface

Science.gov (United States)

Lin, Yu; Wang, Lei; Gao, Jun; Lu, Yichao; Jiang, Suhua; Zeng, Wei

2017-03-01

We experimentally and theoretically demonstrate an ultrathin, broadband, and highly efficient metamaterial-based polarization converter with a metasurface/insulator/metal (MIM) configuration. In such a system, the resonance undergoes a transition from a vertical Fabry-Pérot type to a transverse type as the spacer thickness decreases. By changing the spacer thickness from 1 to 15 mm, the working waveband of this device could be tuned from 10.9-12.9 to 6-8 GHz without compromising the polarization conversion efficiency. Equivalent circuit theory and the transfer matrix method are used for demonstrating the physical mechanism of our device.

Detecting Super-Thin Clouds With Polarized Light

Science.gov (United States)

Sun, Wenbo; Videen, Gorden; Mishchenko, Michael I.

2014-01-01

We report a novel method for detecting cloud particles in the atmosphere. Solar radiation backscattered from clouds is studied with both satellite data and a radiative transfer model. A distinct feature is found in the angle of linear polarization of solar radiation that is backscattered from clouds. The dominant backscattered electric field from the clear-sky Earth-atmosphere system is nearly parallel to the Earth surface. However, when clouds are present, this electric field can rotate significantly away from the parallel direction. Model results demonstrate that this polarization feature can be used to detect super-thin cirrus clouds having an optical depth of only 0.06 and super-thin liquid water clouds having an optical depth of only 0.01. Such clouds are too thin to be sensed using any current passive satellite instruments.

Research and development on optically pumped polarized ion sources. Technical progress report, July 1, 1985-June 30, 1986

International Nuclear Information System (INIS)

Anderson, L.W.

1986-07-01

The development of an optically pumped polarized 23 Na target is discussed. The three categories of research are: (1) electron spin relaxation of the 23 Na due to wall collisions; (2) effects of radiation trapping on the polarization that can be produced in an alkali target by optical pumping; and (3) the effects of spin exchange collisions in the polarization of a fast H 0 beam formed by charge transfer as an H + beam passes through a polarized alkali target. 90 refs., 7 figs

Resonance-inclined optical nuclear spin polarization of liquids in diamond structures

Science.gov (United States)

Chen, Q.; Schwarz, I.; Jelezko, F.; Retzker, A.; Plenio, M. B.

2016-02-01

Dynamic nuclear polarization (DNP) of molecules in a solution at room temperature has the potential to revolutionize nuclear magnetic resonance spectroscopy and imaging. The prevalent methods for achieving DNP in solutions are typically most effective in the regime of small interaction correlation times between the electron and nuclear spins, limiting the size of accessible molecules. To solve this limitation, we design a mechanism for DNP in the liquid phase that is applicable for large interaction correlation times. Importantly, while this mechanism makes use of a resonance condition similar to solid-state DNP, the polarization transfer is robust to a relatively large detuning from the resonance due to molecular motion. We combine this scheme with optically polarized nitrogen-vacancy (NV) center spins in nanodiamonds to design a setup that employs optical pumping and is therefore not limited by room temperature electron thermal polarization. We illustrate numerically the effectiveness of the model in a flow cell containing nanodiamonds immobilized in a hydrogel, polarizing flowing water molecules 4700-fold above thermal polarization in a magnetic field of 0.35 T, in volumes detectable by current NMR scanners.

Laser-driven polarized hydrogen and deuterium internal targets

International Nuclear Information System (INIS)

Jones, C.E.; Fedchak, J.A.; Kowalczyk, R.S.

1995-01-01

After completing comprehensive tests of the performance of the source with both hydrogen and deuterium gas, we began tests of a realistic polarized deuterium internal target. These tests involve characterizing the atomic polarization and dissociation fraction of atoms in a storage cell as a function of flow and magnetic field, and making direct measurements of the average nuclear tensor polarization of deuterium atoms in the storage cell. Transfer of polarization from the atomic electron to the nucleus as a result of D-D spin-exchange collisions was observed in deuterium, verifying calculations suggesting that high vector polarization in both hydrogen and deuterium can be obtained in a gas in spin temperature equilibrium without inducing RF transitions between the magnetic substates. In order to improve the durability of the system, the source glassware was redesigned to simplify construction and installation and eliminate stress points that led to frequent breakage. Improvements made to the nuclear polarimeter, which used the low energy 3 H(d,n) 4 He reaction to analyze the tensor polarization of the deuterium, included installing acceleration lenses constructed of wire mesh to improve pumping conductance, construction of a new holding field coil, and elimination of the Wien filter from the setup. These changes substantially simplified operation of the polarimeter and should have reduced depolarization in collisions with the wall. However, when a number of tests failed to show an improvement of the nuclear polarization, it was discovered that extended operation of the system with a section of teflon as a getter for potassium caused the dissociation fraction to decline with time under realistic operating conditions, suggesting that teflon may not be a suitable material to eliminate potassium from the target. We are replacing the teflon surfaces with drifilm-coated ones and plan to continue tests of the polarized internal target in this configuration

In situ scanning tunneling microscope tip treatment device for spin polarization imaging

Science.gov (United States)

Li, An-Ping [Oak Ridge, TN; Jianxing, Ma [Oak Ridge, TN; Shen, Jian [Knoxville, TN

2008-04-22

A tip treatment device for use in an ultrahigh vacuum in situ scanning tunneling microscope (STM). The device provides spin polarization functionality to new or existing variable temperature STM systems. The tip treatment device readily converts a conventional STM to a spin-polarized tip, and thereby converts a standard STM system into a spin-polarized STM system. The tip treatment device also has functions of tip cleaning and tip flashing a STM tip to high temperature (>2000.degree. C.) in an extremely localized fashion. Tip coating functions can also be carried out, providing the tip sharp end with monolayers of coating materials including magnetic films. The device is also fully compatible with ultrahigh vacuum sample transfer setups.

Role of polarizer-tilting-angle in zero-field spin-transfer nano-oscillators with perpendicular anisotropy

Energy Technology Data Exchange (ETDEWEB)

Gonzalez-Fuentes, C.; Gallardo, R. A., E-mail: rodolfo.gallardo@usm.cl; Landeros, P. [Departamento de Física, Universidad Técnica Federico Santa María, Avenida España 1680, 2390123 Valparaíso (Chile)

2015-10-05

An analytical model for studying the stability of a single domain ferromagnetic layer under the influence of a spin-polarized current is presented. The theory is applied to bias-field-free nano-oscillators with perpendicular anisotropy, which allows to obtain a polarizer-angle vs. current phase diagram that describes the stability of magnetic states. Explicit formulae for the critical current densities unveil the influence of the relative orientation between free and polarizer layers, allowing the emergence of precessional steady-states, and also the possibility to reduce the magnitude of the threshold current density to produce microwave oscillations. It is shown that oscillating steady-states arise in a broad angular region, and the dependence of their boundaries is fully specified by the model. The reliability of the analytical results has been corroborated by comparison to numerical calculations. Such structures are currently under intense research because of remarkable properties offering new prospects for microwave applications in communication technologies.

Graphene-assisted near-field radiative heat transfer between corrugated polar materials

International Nuclear Information System (INIS)

Liu, X. L.; Zhang, Z. M.

2014-01-01

Graphene has attracted great attention in nanoelectronics, optics, and energy harvesting. Here, the near-field radiative heat transfer between graphene-covered corrugated silica is investigated based on the exact scattering theory. It is found that graphene can improve the radiative heat flux between silica gratings by more than one order of magnitude and alleviate the performance sensitivity to lateral shift. The underlying mechanism is mainly attributed to the improved photon tunneling of modes away from phonon resonances. Besides, coating with graphene leads to nonlocal radiative transfer that breaks Derjaguin's proximity approximation and enables corrugated silica to outperform bulk silica in near-field radiation.

W-Band Circularly Polarized TE11 Mode Transducer

Science.gov (United States)

Zhan, Mingzhou; He, Wangdong; Wang, Lei

2018-06-01

This paper presents a balanced sidewall exciting approach to realize the circularly polarized TE11 mode transducer. We used a voltage vector transfer matrix to establish the relationship between input and output vectors, then we analyzed amplitude and phase errors to estimate the isolation of degenerate mode. A mode transducer with a sidewall exciter was designed based on the results. In the 88-100 GHz frequency range, the simulated axial ratio is less than 1.05 and the isolation of linearly polarization TE11 mode is higher than 30 dBc. In back-to-back measurements, the return loss is generally greater than 20 dB with a typical insertion loss of 1.2 dB. Back-to-back transmission measurements are in excellent agreement with simulations.

Dynamics of the polar ionosphere structure disturbance in the Svalgaard-Mansurov effect

International Nuclear Information System (INIS)

Osipov, N.K.; Mozhaev, A.M.; Larina, T.N.; Ponomarev, Yu.N.

1988-01-01

Nonstationary disturbance model of the ionsphere of polar caps caused by change of B y component sign of interplanetary magnetic field is considered. It is shown that nonstationary convection transfer of ionospheric plasma represents the main and the most fast mechanism regulating reconstruction of ionosphere structure in polar caps during magnetosphere substorms, caused by the change of B y sign. Calculations show that characteristic time of sufficient change of ionosphere structure at ∼1500 km distances is on the order of 10-25 min

Hardness and softness reactivity kernels within the spin-polarized density-functional theory

International Nuclear Information System (INIS)

Chamorro, Eduardo; De Proft, Frank; Geerlings, Paul

2005-01-01

Generalized hardness and softness reactivity kernels are defined within a spin-polarized density-functional theory (SP-DFT) conceptual framework. These quantities constitute the basis for the global, local (i.e., r-position dependent), and nonlocal (i.e., r and r ' -position dependents) indices devoted to the treatment of both charge-transfer and spin-polarization processes in such a reactivity framework. The exact relationships between these descriptors within a SP-DFT framework are derived and the implications for chemical reactivity in such context are outlined

Investigating dust trapping in transition disks with millimeter-wave polarization

Science.gov (United States)

Pohl, A.; Kataoka, A.; Pinilla, P.; Dullemond, C. P.; Henning, Th.; Birnstiel, T.

2016-08-01

Context. Spatially resolved polarized (sub-)mm emission has been observed for example in the protoplanetary disk around HL Tau. Magnetically aligned grains are commonly interpreted as the source of polarization. However, self-scattering by large dust grains with a high enough albedo is another polarization mechanism, which is becoming a compelling method independent of the spectral index to constrain the dust grain size in protoplanetary disks. Aims: We study the dust polarization at mm wavelengths in the dust trapping scenario proposed for transition disks, when a giant planet opens a gap in the disk. We investigate the characteristic polarization patterns and their dependence on disk inclination, dust size evolution, planet position, and observing wavelength. Methods: We combine two-dimensional hydrodynamical simulations of planet-disk interactions with self-consistent dust growth models. These size-dependent dust density distributions are used for follow-up three-dimensional radiative transfer calculations to predict the polarization degree at ALMA bands due to scattered thermal emission. Results: Dust self-scattering has been proven to be a viable mechanism for producing polarized mm-wave radiation. We find that the polarization pattern of a disk with a planetary gap after 1 Myr of dust evolution shows a distinctive three-ring structure. Two narrow inner rings are located at the planet gap edges. A third wider ring of polarization is situated in the outer disk beyond 100 au. For increasing observing wavelengths, all three rings change their position slightly, where the innermost and outermost rings move inward. This distance is detectable when comparing the results at ALMA bands 3, 6, and 7. Within the highest polarized intensity regions the polarization vectors are oriented in the azimuthal direction. For an inclined disk there is an interplay between polarization originating from a flux gradient and inclination-induced quadrupole polarization. For

Polarization of lanthanum nucleus by dynamic polarization method

International Nuclear Information System (INIS)

Adachi, Toshikazu; Ishimoto, Shigeru; Masuda, Yasuhiro; Morimoto, Kimio

1989-01-01

Preliminary studies have been carried out concerning the application of a dynamic polarization method to polarizing lanthanum fluoride single crystal to be employed as target in experiments with time reversal invariance. The present report briefly outlines the dynamic polarization method and describes some preliminary studies carried out so far. Dynamic polarization is of particular importance because no techniques are currently available that can produce highly polarized static nucleus. Spin interaction between electrons and protons (nuclei) plays a major role in the dynamic polarization method. In a thermal equilibrium state, electrons are polarized almost completely while most protons are not polarized. Positively polarized proton spin is produced by applying microwave to this system. The most hopeful candidate target material is single crystal of LaF 3 containing neodymium because the crystal is chemically stable and easy to handle. The spin direction is of great importance in experiments with time reversal invariance. The spin of neutrons in the target can be cancelled by adjusting the external magnetic field applied to a frozen polarized target. In a frozen spin state, the polarity decreases slowly with a relaxation time that depends on the external magnetic field and temperature. (N.K.)

Polarization-Dependent Measurements of Molecular Super Rotors with Oriented Angular Momenta

Science.gov (United States)

Murray, Matthew J.; Toro, Carlos; Liu, Qingnan; Mullin, Amy S.

2014-05-01

Controlling molecular motion would enable manipulation of energy flow between molecules. Here we have used an optical centrifuge to investigate energy transfer between molecular super rotors with oriented angular momenta. The polarizable electron cloud of the molecules interacts with the electric field of linearly polarized light that angularly accelerates over the time of the optical pulse. This process drives molecules into high angular momentum states that are oriented with the optical field and have energies far from equilibrium. High resolution transient IR spectroscopy reveals the dynamics of collisional energy transfer for these super excited rotors. The results of this study leads to a more fundamental understanding of energy balance in non-equilibrium environments and the physical and chemical properties of gases in a new regime of energy states. Results will be presented for several super rotor species including carbon monoxide, carbon dioxide, and acetylene. Polarization-dependent measurements reveal the extent to which the super rotors maintain spatial orientation of high angular momentum states.

Polarized neutrons

International Nuclear Information System (INIS)

Williams, W.G.

1988-01-01

The book on 'polarized neutrons' is intended to inform researchers in condensed matter physics and chemistry of the diversity of scientific problems that can be investigated using polarized neutron beams. The contents include chapters on:- neutron polarizers and instrumentation, polarized neutron scattering, neutron polarization analysis experiments and precessing neutron polarization. (U.K.)

Effect of solvent polarity and temperature on the spectral and thermodynamic properties of exciplexes of 1-cyanonaphthalene with hexamethylbenzene in organic solvents

Energy Technology Data Exchange (ETDEWEB)

Asim, Sadia [Institute of Physical and Theoretical Chemistry, Graz University of Technology, Stremaryrgasse 9, A-8010 Graz (Austria); Department of Chemistry and Biochemistry, University of Agriculture, Faisalabad (Pakistan); Mansha, Asim [Institute of Physical and Theoretical Chemistry, Graz University of Technology, Stremaryrgasse 9, A-8010 Graz (Austria); Department of Chemistry, Government College University, Faisalabad (Pakistan); Grampp, Günter, E-mail: grampp@tugraz.at [Institute of Physical and Theoretical Chemistry, Graz University of Technology, Stremaryrgasse 9, A-8010 Graz (Austria); Landgraf, Stephan [Institute of Physical and Theoretical Chemistry, Graz University of Technology, Stremaryrgasse 9, A-8010 Graz (Austria); Zahid, Muhammad [Institute of Physical and Theoretical Chemistry, Graz University of Technology, Stremaryrgasse 9, A-8010 Graz (Austria); Department of Chemistry and Biochemistry, University of Agriculture, Faisalabad (Pakistan); Bhatti, Ijaz Ahmad [Department of Chemistry and Biochemistry, University of Agriculture, Faisalabad (Pakistan)

2014-09-15

Study of the effect of solvent polarity and temperature is done on the exciplex emission spectra of 1-cyanonaphthalene with hexamethylbenzene. Exciplex system is studied in the range of partially polar solvents and in solvent mixture of propyl acetate and butyronitrile. The unique feature of this solvent mixture is that only the solvent polarity changes (6.0≤ε{sub s}≤24.7) with the change in the mole fraction of solvents whereas the solvent viscosity and refractive index remains unaffected. Thermodynamic properties are calculated according to the models developed by Weller and Kuzmin. Fluorescence lifetimes for both the fluorophore as well as the exciplex are evaluated in all used solvents. Exciplex energetics as a function of solvent polarity and temperature are also discussed. Kuzmin model of self-consistent polarization is used for the explanation of the exciplex emission spectra. The effects of solvent polarity and temperature on energy of zero–zero transitions (hv{sub 0}{sup /}), Huang–Rhys factor (S), Gauss broadening of vibronic level (σ) and the dominant high-frequency vibration (hν{sub ν}) are investigated. The strong dependence of exciplex stability and energetics upon the solvent polarity and temperature are observed. Full charge transfer exciplexes were observed in solvents of all polarities and stronger exciplex with large emission intensities were found in solvents of low polarities but with the increase in solvent polarity the exciplex becomes weak and they dissociate fastly into radical ion pairs. The kinetic model of Kuzmin was observed to reduce into the Weller kinetic model for this exciplex system with ∆G{sub ET} = −0.22 eV and the spectral shift, h∆ν>0.2 eV. - Highlights: • Exciplex formed as a result of mixing of charge transfer and locally excited states. • Effect of solvents polarity and temperature on the exciplex stability and thermodynamics. • Solvent polarity will decide the formation of contact radical ion pair

Multiangular hyperspectral investigation of polarized light in case 2 waters

Science.gov (United States)

Tonizzo, A.; Zhou, J.; Gilerson, A.; Chowdhary, J.; Gross, B.; Moshary, F.; Ahmed, S.

2009-09-01

The focus of this work is on the dependence of in situ hyperspectral and multiangular polarized data on the size distribution and refractive index of the suspended particles. Underwater polarization measurements were obtained using a polarimeter developed at the Optical Remote Sensing Laboratory of the City College of New York, NY. The degree of polarization (DOP) of the underwater light field in coastal environments was measured and the water-leaving polarized radiance was derived. In-water optical properties were also measured with an ac-9 (WET Labs). Absorption and attenuation spectra are then used to derive information on the dissolved and suspend components in the water medium which are used in a vector radiative transfer code which provides the upwelling radiance. The model was run for various values of the refractive index of mineral particles until the modeled DOP matched the measured one. The relationship between the intensity of the maximum of the DOP and both the refractive index of the mineral particles and the shapes of their size distributions is analyzed in detail.

Realization of a broad band neutron spin filter with compressed, polarized 3He gas

International Nuclear Information System (INIS)

Surkau, R.; Otten, E.W.; Steiner, M.; Tasset, F.; Trautmann, N.

1997-01-01

The strongly spin dependent absorption of neutrons in nuclear spin polarized 3 -2pt vector He opens the possibility to polarize beams of thermal and epithermal neutrons. An effective 3 He neutron spin filter (NSF) requires high 3 He nuclear polarization as well as a filter thickness corresponding to a gas amount of the order of 1 bar l. We realized such a filter using direct optical pumping of metastable 3 He * atoms in a 3 He plasma at 1 mbar. Metastable exchange scattering transfers the angular momentum to the whole ensemble of 3 He atoms. At present 3 x 10 18 3 He-atoms/s are polarized up to 64%. Subsequent polarization preserving compression by a two stage compressor system enables to prepare NSF cells of about 300 cm 3 volume with 3 bar of polarized 3 He within 2 h. 3 He polarizations up to 53% were measured in a cell with a filter length of about 15 cm. By this cell a thermal neutron beam from the Mainz TRIGA reactor was polarized. A wavelength selective polarization analysis by means of Bragg scattering revealed a neutron polarization of 84% at a total transmission of 12% for a neutron wavelength of 1 A. (orig.)

Polarized recombination of acoustically transported carriers in GaAs nanowires

Science.gov (United States)

Möller, Michael; Hernández-Mínguez, Alberto; Breuer, Steffen; Pfüller, Carsten; Brandt, Oliver; de Lima, Mauricio M.; Cantarero, Andrés; Geelhaar, Lutz; Riechert, Henning; Santos, Paulo V.

2012-05-01

The oscillating piezoelectric field of a surface acoustic wave (SAW) is employed to transport photoexcited electrons and holes in GaAs nanowires deposited on a SAW delay line on a LiNbO3 crystal. The carriers generated in the nanowire by a focused light spot are acoustically transferred to a second location where they recombine. We show that the recombination of the transported carriers occurs in a zinc blende section on top of the predominant wurtzite nanowire. This allows contactless control of the linear polarized emission by SAWs which is governed by the crystal structure. Additional polarization-resolved photoluminescence measurements were performed to investigate spin conservation during transport.

Induced polarization of Λ (1116) in kaon electroproduction

Science.gov (United States)

Gabrielyan, M.; Raue, B. A.; Carman, D. S.; Park, K.; Adhikari, K. P.; Adikaram, D.; Amaryan, M. J.; Anefalos Pereira, S.; Avakian, H.; Ball, J.; Baltzell, N. A.; Battaglieri, M.; Baturin, V.; Bedlinskiy, I.; Biselli, A. S.; Bono, J.; Boiarinov, S.; Briscoe, W. J.; Brooks, W. K.; Burkert, V. D.; Cao, T.; Celentano, A.; Chandavar, S.; Charles, G.; Colaneri, L.; Cole, P. L.; Contalbrigo, M.; Cortes, O.; Crede, V.; D'Angelo, A.; Dashyan, N.; De Vita, R.; De Sanctis, E.; Deur, A.; Djalali, C.; Doughty, D.; Dupre, R.; El Fassi, L.; Eugenio, P.; Fedotov, G.; Fegan, S.; Fleming, J. A.; Forest, T. A.; Garillon, B.; Gevorgyan, N.; Ghandilyan, Y.; Gilfoyle, G. P.; Giovanetti, K. L.; Girod, F. X.; Goetz, J. T.; Golovatch, E.; Gothe, R. W.; Griffioen, K. A.; Guidal, M.; Guo, L.; Hafidi, K.; Hakobyan, H.; Hattawy, M.; Hicks, K.; Ho, D.; Holtrop, M.; Hughes, S. M.; Ilieva, Y.; Ireland, D. G.; Ishkhanov, B. S.; Jenkins, D.; Jiang, H.; Jo, H. S.; Joo, K.; Keller, D.; Khandaker, M.; Kim, W.; Klein, F. J.; Koirala, S.; Kubarovsky, V.; Kuhn, S. E.; Kuleshov, S. V.; Lenisa, P.; Levine, W. I.; Livingston, K.; MacGregor, I. J. D.; Mayer, M.; McKinnon, B.; Meyer, C. A.; Mestayer, M. D.; Mirazita, M.; Mokeev, V.; Moody, C. I.; Moutarde, H.; Movsisyan, A.; Munevar, E.; Munoz Camacho, C.; Nadel-Turonski, P.; Niccolai, S.; Niculescu, G.; Osipenko, M.; Pappalardo, L. L.; Paremuzyan, R.; Pasyuk, E.; Peng, P.; Phelps, W.; Phillips, J. J.; Pisano, S.; Pogorelko, O.; Pozdniakov, S.; Price, J. W.; Procureur, S.; Protopopescu, D.; Rimal, D.; Ripani, M.; Rizzo, A.; Sabatié, F.; Salgado, C.; Schott, D.; Schumacher, R. A.; Simonyan, A.; Smith, G. D.; Sober, D. I.; Sokhan, D.; Stepanyan, S. S.; Stepanyan, S.; Strakovsky, I. I.; Strauch, S.; Sytnik, V.; Tang, W.; Ungaro, M.; Vlassov, A. V.; Voskanyan, H.; Voutier, E.; Walford, N. K.; Watts, D. P.; Wei, X.; Weinstein, L. B.; Zachariou, N.; Zana, L.; Zhang, J.; Zonta, I.; CLAS Collaboration

2014-09-01

We have measured. the induced polarization of the Λ(1116) in the reaction ep →e'K+Λ, detecting the scattered e' and K+ in the final state along with the proton from the decay Λ →pπ-. The present study used the CEBAF Large Acceptance Spectrometer (CLAS), which allowed for a large kinematic acceptance in invariant energy W (1.6≤W≤2.7 GeV) and covered the full range of the kaon production angle at an average momentum transfer Q2=1.90GeV2. In this experiment a 5.50-GeV electron beam was incident upon an unpolarized liquid-hydrogen target. We have mapped out the W and kaon production angle dependencies of the induced polarization and found striking differences from photoproduction data over most of the kinematic range studied. However, we also found that the induced polarization is essentially Q2 independent in our kinematic domain, suggesting that somewhere below the Q2 covered here there must be a strong Q2 dependence. Along with previously published photo- and electroproduction cross sections and polarization observables, these data are needed for the development of models, such as effective field theories, and as input to coupled-channel analyses that can provide evidence of previously unobserved s-channel resonances.

Recursive polarization of nuclear spins in diamond at arbitrary magnetic fields

International Nuclear Information System (INIS)

Pagliero, Daniela; Laraoui, Abdelghani; Henshaw, Jacob D.; Meriles, Carlos A.

2014-01-01

We introduce an alternate route to dynamically polarize the nuclear spin host of nitrogen-vacancy (NV) centers in diamond. Our approach articulates optical, microwave, and radio-frequency pulses to recursively transfer spin polarization from the NV electronic spin. Using two complementary variants of the same underlying principle, we demonstrate nitrogen nuclear spin initialization approaching 80% at room temperature both in ensemble and single NV centers. Unlike existing schemes, our approach does not rely on level anti-crossings and is thus applicable at arbitrary magnetic fields. This versatility should prove useful in applications ranging from nanoscale metrology to sensitivity-enhanced NMR

Are digital images good enough? A comparative study of conventional film-screen vs digital radiographs on printed images of total hip replacement

Energy Technology Data Exchange (ETDEWEB)

Eklund, K.; Jonsson, K.; Lindblom, G.; Lundin, B.; Sanfridsson, J.; Sloth, M. [Department of Radiology, Center for Medical Imaging and Physiology, Lund University Hospital, 22185, Lund (Sweden); Sivberg, B. [Department of Nursing, Faculty of Medicine, Lund University, P.O. Box 157, 22100, Lund (Sweden)

2004-05-01

The aim of this study was to evaluate the inter- and intra-observer variability and to find differences in diagnostic safety between digital and analog technique in diagnostic zones around hip prostheses. In 80 patients who had had a total hip replacement (THR) for more than 2 years, a conventional image and a digital image were taken. Gruen's model of seven distinct regions of interest was used for evaluations. Five experienced radiologists observed the seven regions and noted in a protocol the following distances: stem-cement; cement-bone; and stem-bone. All images were printed on hard copies and were read twice. Weighted kappa, {kappa}{sub w}, analyses were used. The two most frequently loosening regions, stem-cement region 1 and cement-bone region 7, were closely analyzed. In region 1 the five observers had an agreement of 86.75-97.92% between analog and digital images in stem-cement, which is a varied {kappa}{sub w} 0.29-0.71. For cement-bone region 7 an agreement of 87.21-90.45% was found, which is a varied {kappa}{sub w} of 0.48-0.58. All the kappa values differ significantly from nil. The result shows that digital technique is as good as analog radiographs for diagnosing possible loosening of hip prostheses. (orig.)

Effects of multiple scattering and atmospheric aerosol on the polarization of the twilight sky

International Nuclear Information System (INIS)

Ugolnikov, Oleg S.; Postylyakov, Oleg V.; Maslov, Igor A.

2004-01-01

The paper presents a review of a number of wide-angle polarization CCD-measurements of the twilight sky in V and R color bands with effective wavelengths 550 and 700nm. The basic factors affecting (usually decreasing) the polarization of the twilight sky are the atmospheric aerosol scattering and multiple scattering. These effects were distinguished from each other, and a method of multiple-scattering separation is discussed. The results are compared with the data of numerical simulation of radiative transfer in the atmosphere for different aerosol models. The whole twilight period is divided into different stages with different mechanisms forming the twilight-sky polarization properties

Workshop on polarized neutron filters and polarized pulsed neutron experiments

International Nuclear Information System (INIS)

Itoh, Shinichi

2004-07-01

The workshop was held in KEK by thirty-three participants on April 26, 2004. The polarized neutron filter method was only discussed. It consists of three parts; the first part was discussed on the polarized neutron methods, the second part on the polarized neutron experiments and the third on the pulse neutron spectrometer and polarized neutron experiments. The six papers were presented such as the polarized 3 He neutron spin filter, neutron polarization by proton polarized filter, soft master and neutron scattering, polarized neutron in solid physics, polarization experiments by chopper spectroscope and neutron polarization system in superHRPD. (S.Y.)

Electrochemical behavior of uranyl in anhydrous polar organic media

Energy Technology Data Exchange (ETDEWEB)

Burn, Adam G.; Nash, Kenneth L. [Washington State Univ., Pullmann, WA (United States). Dept. of Chemistry

2017-09-01

Weak complexes between pentavalent and hexavalent actinyl cations have been reported to exist in acidic, non-complexing high ionic strength aqueous media. Such ''cation-cation complexes'' were first identified in the context of actinide-actinide redox reactions in acidic aqueous media relevant to solvent extraction-based separation systems, hence their characterization is of potential interest for advanced nuclear fuel reprocessing. This chemistry could be relevant to efforts to develop advanced actinide separations based on the upper oxidation states of americium, which are of current interest. In the present study, the chemical behavior of pentavalent uranyl was examined in non-aqueous, aprotic polar organic solvents (propylene carbonate and acetonitrile) to determine whether UO{sub 2}{sup +} cations generated at the reducing working electrode surface would interact with the UO{sub 2}{sup 2+} cations in the bulk phase to form cation-cation complexes in such media. In magnesium perchlorate media, the electrolyte adsorbed onto the working electrode surface and interfered with the uranyl reduction/diffusion process through an ECE (electron transfer/chemical reaction/electron transfer) mechanism. In parallel studies of uranyl redox behavior in tetrabutylammonium hexafluorophosphate solutions, an EC (electron transfer/chemical reaction) mechanism was observed in the cyclic voltammograms. Ultimately, no conclusive electrochemical evidence demonstrated uranyl cation-cation interactions in the non-aqueous, aprotic polar organic solvent solutions, though the results reported do not completely rule out the presence of UO{sub 2}{sup +}.UO{sub 2}{sup 2+} complexes.

Investigation of. epsilon. sub 1 and the sup 3 P sub J phase shifts in the n-p system by the measurement of polarization transfer coefficients in p-d elastic scattering

Energy Technology Data Exchange (ETDEWEB)

Clajus, M.; Egun, P.M.; Grueebler, W.; Hautle, P. (Eidgenoessische Technische Hochschule, Zurich (Switzerland). Inst. fuer Mittelenergiephysik); Kretschmer, W.; Rauscher, A.; Schuster, W.; Weidmann, R.; Haller, M. (Erlangen-Nuernberg Univ., Erlangen (Germany, F.R.). Physikalisches Inst.); Bruno, M.; Cannata, F.; D' Agostino, M. (Istituto Nazionale di Fisica Nucleare, Bologna (Italy) Bologna Univ. (Italy). Dipt. di Fisica); Slaus, I. (Institut Rudjer Boskovic, Zagreb (Yugoslavia)); Schmelzbach, P.A. (Paul Scherrer Inst., Villigen (Switzerland)); Vuaridel, B. (Michigan Univ., Ann Arbor (USA)); Sperisen, F. (Indiana Univ., Bloomington (USA). Cyclotron Facility); Witala, H.; Cornelius, T.; Gloeckle, W. (Bochum Univ. (Germany, F.R.))

1990-02-01

The {sup 3}S{sub 1}-{sup 3}D{sub 1} mixing parameter {epsilon}{sub 1} and the {sup 3}P{sub J} phase shifts in the N-N system at low energy are investigated in the three nucleon system. The sensitivity of polarization transfer coefficients in p-d elastic scattering is determined by rigorous Faddeev calculations using Paris and Bonn potentials. The experimental results of K{sub y}sup(y') favours the tensor force component of the Bonn A potential. (orig.).

Transfer matrix approach for the Kerr and Faraday rotation in layered nanostructures.

Science.gov (United States)

Széchenyi, Gábor; Vigh, Máté; Kormányos, Andor; Cserti, József

2016-09-21

To study the optical rotation of the polarization of light incident on multilayer systems consisting of atomically thin conductors and dielectric multilayers we present a general method based on transfer matrices. The transfer matrix of the atomically thin conducting layer is obtained using the Maxwell equations. We derive expressions for the Kerr (Faraday) rotation angle and for the ellipticity of the reflected (transmitted) light as a function of the incident angle and polarization of the light. The method is demonstrated by calculating the Kerr (Faraday) angle for bilayer graphene in the quantum anomalous Hall state placed on the top of dielectric multilayers. The optical conductivity of the bilayer graphene is calculated in the framework of a four-band model.

Dual descriptors within the framework of spin-polarized density functional theory.

Science.gov (United States)

Chamorro, E; Pérez, P; Duque, M; De Proft, F; Geerlings, P

2008-08-14

Spin-polarized density functional theory (SP-DFT) allows both the analysis of charge-transfer (e.g., electrophilic and nucleophilic reactivity) and of spin-polarization processes (e.g., photophysical changes arising from electron transitions). In analogy with the dual descriptor introduced by Morell et al. [J. Phys. Chem. A 109, 205 (2005)], we introduce new dual descriptors intended to simultaneously give information of the molecular regions where the spin-polarization process linking states of different multiplicity will drive electron density and spin density changes. The electronic charge and spin rearrangement in the spin forbidden radiative transitions S(0)-->T(n,pi(*)) and S(0)-->T(pi,pi(*)) in formaldehyde and ethylene, respectively, have been used as benchmark examples illustrating the usefulness of the new spin-polarization dual descriptors. These quantities indicate those regions where spin-orbit coupling effects are at work in such processes. Additionally, the qualitative relationship between the topology of the spin-polarization dual descriptors and the vertical singlet triplet energy gap in simple substituted carbene series has been also discussed. It is shown that the electron density and spin density rearrangements arise in agreement with spectroscopic experimental evidence and other theoretical results on the selected target systems.

Spectral element method for vector radiative transfer equation

International Nuclear Information System (INIS)

Zhao, J.M.; Liu, L.H.; Hsu, P.-F.; Tan, J.Y.

2010-01-01

A spectral element method (SEM) is developed to solve polarized radiative transfer in multidimensional participating medium. The angular discretization is based on the discrete-ordinates approach, and the spatial discretization is conducted by spectral element approach. Chebyshev polynomial is used to build basis function on each element. Four various test problems are taken as examples to verify the performance of the SEM. The effectiveness of the SEM is demonstrated. The h and the p convergence characteristics of the SEM are studied. The convergence rate of p-refinement follows the exponential decay trend and is superior to that of h-refinement. The accuracy and efficiency of the higher order approximation in the SEM is well demonstrated for the solution of the VRTE. The predicted angular distribution of brightness temperature and Stokes vector by the SEM agree very well with the benchmark solutions in references. Numerical results show that the SEM is accurate, flexible and effective to solve multidimensional polarized radiative transfer problems.

IOCCG Report Number 16, 2015 Ocean Colour Remote Sensing in Polar Seas . Chapter 2; The Polar Environment: Sun, Clouds, and Ice

Science.gov (United States)

Comiso, Josefino C.; Perovich, Don; Stamnes, Knut; Stuart, Venetia (Editor)

2015-01-01

The polar regions are places of extremes. There are months when the regions are enveloped in unending darkness, and months when they are in continuous daylight. During the daylight months the sun is low on the horizon and often obscured by clouds. In the dark winter months temperatures are brutally cold, and high winds and blowing snow are common. Even in summer, temperatures seldom rise above 0degC. The cold winter temperatures cause the ocean to freeze, forming sea ice. This sea ice cover acts as a barrier limiting the transfer of heat, moisture, and momentum between the atmosphere and the ocean. It also greatly complicates the optical signature of the surface. Taken together, these factors make the polar regions a highly challenging environment for optical remote sensing of the ocean.

Intramolecular, Exciplex-Mediated, Proton-Coupled, Charge-Transfer Processes in N,N-Dimethyl-3-(1-pyrenyl)propan-1-ammonium Cations: Influence of Anion, Solvent Polarity, and Temperature.

Science.gov (United States)

Safko, Trevor M; Faleiros, Marcelo M; Atvars, Teresa D Z; Weiss, Richard G

2016-06-16

An intramolecular exciplex-mediated, proton-coupled, charge-transfer (PCCT) process has been investigated for a series of N,N-dimethyl-3-(1-pyrenyl)propan-1-ammonium cations with different anions (PyS) in solvents of low to intermediate polarity over a wide temperature range. Solvent mediates both the equilibrium between conformations of the cation that place the pyrenyl and ammonium groups in proximity (conformation C) or far from each other (conformation O) and the ability of the ammonium group to transfer a proton adiabatically in the PyS excited singlet state. Thus, exciplex emission, concurrent with the PCCT process, was observed only in hydrogen-bond accepting solvents of relatively low polarity (tetrahydrofuran, ethyl acetate, and 1,4-dioxane) and not in dichloromethane. From the exciplex emission and other spectroscopic and thermodynamic data, the acidity of the ammonium group in conformation C of the excited singlet state of PyS (pKa*) has been estimated to be ca. -3.4 in tetrahydrofuran. The ratios between the intensities of emission from the exciplex and the locally excited state (IEx/ILE) appear to be much more dependent on the nature of the anion than are the rates of exciplex formation and decay, although the excited state data do not provide a quantitative measure of the anion effect on the C-O equilibrium. The activation energies associated with exciplex formation in THF are calculated to be 0.08 to 0.15 eV lower than for the neutral amine, N,N-dimethyl-3-(1-pyrenyl)propan-1-amine. Decay of the exciplexes formed from the deprotonation of PyS is hypothesized to occur through charge-recombination processes. To our knowledge, this is the first example in which photoacidity and intramolecular exciplex formation (i.e., a PCCT reaction) are coupled.

When measured spin polarization is not spin polarization

International Nuclear Information System (INIS)

Dowben, P A; Wu Ning; Binek, Christian

2011-01-01

Spin polarization is an unusually ambiguous scientific idiom and, as such, is rarely well defined. A given experimental methodology may allow one to quantify a spin polarization but only in its particular context. As one might expect, these ambiguities sometimes give rise to inappropriate interpretations when comparing the spin polarizations determined through different methods. The spin polarization of CrO 2 and Cr 2 O 3 illustrate some of the complications which hinders comparisons of spin polarization values. (viewpoint)

On the spectrum and polarization of magnetar flare emission

Science.gov (United States)

Taverna, R.; Turolla, R.

2017-08-01

Bursts and flares are among the distinctive observational manifestations of magnetars, isolated neutron stars endowed with an ultrastrong magnetic field (B ≈ 1014-1015 G). It is believed that these events arise in a hot electron-positron plasma that remains trapped within the closed magnetic field lines. We developed a simple radiative transfer model to simulate magnetar flare emission in the case of a steady trapped fireball. After dividing the fireball surface in a number of plane-parallel slabs, the local spectral and polarization properties are obtained integrating the radiative transfer equations for the two normal modes. We assume that magnetic Thomson scattering is the dominant source of opacity, and neglect contributions from second-order radiative processes, although double-Compton scattering is accounted for in establishing local thermal equilibrium in the fireball atmospheric layers. The observed spectral and polarization properties as measured by a distant observer are obtained by summing the contributions from the patches that are visible for a given viewing geometry by means of a ray-tracing code. The spectra we obtained in the 1-100 keV energy range are thermal and can be described in terms of the superposition of two blackbodies. The blackbody temperature and the emitting area ratio are in broad agreement with the available observations. The predicted linear polarization degree is, in general, greater than 80 per cent over the entire energy range and should be easily detectable by new-generation X-ray polarimeters, such as IXPE, XIPE and eXTP.

A Polarizable and Transferable PHAST CO 2 Potential for Materials Simulation

KAUST Repository

Mullen, Ashley L.; Pham, Tony; Forrest, Katherine A.; Cioce, Christian R.; McLaughlin, Keith; Space, Brian

2013-01-01

Reliable PHAST (Potentials with High Accuracy Speed and Transferability) intermolecular potential energy functions for CO2 have been developed from first principles for use in heterogeneous systems, including one with explicit polarization

Density and speed of sound of lithium bromide with organic solvents: Measurement and correlation

Energy Technology Data Exchange (ETDEWEB)

Zafarani-Moattar, Mohammed Taghi [Department of Physical Chemistry, Faculty of Chemistry, University of Tabriz, Tabriz 51664 (Iran, Islamic Republic of); Research Institute of Fundamental Sciences, Tabriz 51664 (Iran, Islamic Republic of)], E-mail: zafarani47@yahoo.com; Shekaari, Hemayat [Department of Physical Chemistry, Faculty of Chemistry, University of Tabriz, Tabriz 51664 (Iran, Islamic Republic of); Research Institute of Fundamental Sciences, Tabriz 51664 (Iran, Islamic Republic of)

2007-12-15

Densities, {rho}, and speed of sound, u, of the solutions of LiBr with non-aqueous solvents (methanol, ethanol, 2-propanol, acetone, and acetonitrile) having a wide range of dielectric constants were measured at T = 298.15 K. Also, these measurements were made for the system (LiBr + N,N-dimethylacetamide) at T = 323.15 K. For the investigated systems, the limiting values for apparent molar volume, V{sub {phi}}{sup 0}, and the apparent molar isentropic compressibility, {kappa}{sub {phi}}{sup 0}, were obtained from the Redlich-Mayer and an abbreviated form of the Pitzer equations. The Pitzer and NRTL equations were satisfactorily used for the correlation of apparent molar volumes, V{sub {phi}}, and the apparent molar isentropic compressibility, {kappa}{sub {phi}}, values of the studied systems.

Polarization, alignment, and orientation in atomic collisions

CERN Document Server

Andersen, Nils

2017-01-01

This book covers polarization, alignment, and orientation effects in atomic collisions induced by electron, heavy particle, or photon impact. The first part of the book presents introductory chapters on light and particle polarization, experimental and computational methods, and the density matrix and state multipole formalism. Examples and exercises are included. The second part of the book deals with case studies of electron impact and heavy particle excitation, electron transfer, impact ionization, and autoionization. A separate chapter on photo-induced processes by new-generation light sources has been added. The last chapter discusses related topics and applications. Part III includes examples of charge clouds and introductory summaries of selected seminal papers of tutorial value from the early history of the field (1925 – 1975). The book is a significant update to the previous (first) edition, particularly in experimental and computational methods, the inclusion of key results obtained during the pas...

A new approach to radiative transfer theory using Jones's vectors. I

International Nuclear Information System (INIS)

Fymat, A.L.; Vasudevan, R.

1975-01-01

Radiative transfer of partially polarized radiation in an anisotropically scattering, inhomogeneous atmosphere containing arbitrary polydispersion of particles is described using Jones's amplitude vectors and matrices. This novel approach exploits the close analogy between the quantum mechanical states of spin 1/2 systems and the polarization states of electromagnetic radiation described by Jones's vector, and draws on the methodology of such spin 1/2 systems. The complete equivalence between the transport equation for Jones's vectors and the classical radiative transfer equation for Stokes's intensity vectors is demonstrated in two independent ways after deriving the transport equations for the polarization coherency matrices and for the quaternions corresponding to the Jones's vectors. A compact operator formulation of the theory is provided, and used to derive the necessary equations for both a local and a global description of the transport of Jones's vectors. Lastly, the integro-differential equations for the amplitude reflection and transmission matrices are derived, and related to the usual corresponding equations. The present formulation is the most succinct and the most convenient one for both theoretical and experimental studies. It yields a simpler analysis than the classical formulation since it reduces by a factor of two the dimensionality of transfer problems. It preserves information on phases, and thus can be used directly across the entire electromagnetic spectrum without any further conversion into intensities. (Auth.)

Modeling spin selectivity in charge transfer across the DNA/Gold interface

Energy Technology Data Exchange (ETDEWEB)

Behnia, S., E-mail: s.behnia@sci.uut.ac.ir [Department of Physics, Urmia University of Technology, Urmia (Iran, Islamic Republic of); Fathizadeh, S. [Department of Physics, Urmia University of Technology, Urmia (Iran, Islamic Republic of); Akhshani, A. [Department of Physics, Urmia Branch, Islamic Azad University, Urmia (Iran, Islamic Republic of)

2016-09-30

Highlights: • DNA in spintronics is applied. Nearly pure spin current is observed in the system. • A combined spin-polaronic PBH model is proposed for spin transfer in DNA molecule. • Spin Hall effect in DNA due to spin–orbit coupling is verified. • The temperature dependence of Hall conductivity is appeared. • Regions of parameters were determined that polarization of spin current is maximum. - Abstract: Experimental results show that the photoelectrons emitted from the gold substrate due to laser radiation, passe through DNA nanowires with spin-polarized nature. This study proposes the use of chiral DNA molecule in spintronics and information processing. To investigate the spin transfer in DNA molecules, we established a theoretical model based on a combined spin-polaronic Peyrard–Bishop–Holstein model. Accordingly, a nearly pure spin current is appeared. The simultaneous effects of the incident radiation and external magnetic field create characteristic islands corresponding to the pure spin currents, which can be predicted and detected using the multifractal dimensions spectrum. We can verify the spin Hall effect on DNA oligomers through spin–orbit coupling. As such, we can proceed to our significant purpose, which is to create a nearly pure spin current for information transfer and determine the regions of parameter values from which the maximal polarization in spin current emerges.

Effect of polarized radiative transfer on the Hanle magnetic field determination in prominences: Analysis of hydrogen H alpha line observations at Pic-du-Midi

Science.gov (United States)

Bommier, V.; Deglinnocenti, E. L.; Leroy, J. L.; Sahal-Brechot, S.

1985-01-01

The linear polarization of the Hydrogen H alpha line of prominences has been computed, taking into account the effect of a magnetic field (Hanle effect), of the radiative transfer in the prominence, and of the depolarization due to collisions with the surrounding electrons and protons. The corresponding formalisms are developed in a forthcoming series of papers. In this paper, the main features of the computation method are summarized. The results of computation have been used for interpretation in terms of magnetic field vector measurements from H alpha polarimetric observations in prominences performed at Pic-du-Midi coronagraph-polarimeter. Simultaneous observations in one optically thin line (He I D(3)) and one optically thick line (H alpha) give an opportunity for solving the ambiguity on the field vector determination.

Solid state nuclear magnetic resonance studies of cross polarization from quadrupolar nuclei

Energy Technology Data Exchange (ETDEWEB)

De Paul, Susan M. [Univ. of California, Berkeley, CA (United States)

1997-08-01

The development of solid-state Nuclear Magnetic Resonance (NMR) has, to a large extent, focused on using spin-1/2 nuclei as probes to investigate molecular structure and dynamics. For such nuclei, the technique of cross polarization is well-established as a method for sensitivity enhancement. However, over two-thirds of the nuclei in the periodic table have a spin-quantum number greater than one-half and are known as quadrupolar nuclei. Such nuclei are fundamental constituents of many inorganic materials including minerals, zeolites, glasses, and gels. It is, therefore, of interest to explore the extent to which polarization can be transferred from quadrupolar nuclei. In this dissertation, solid-state NMR experiments involving cross polarization from quadrupolar nuclei to spin-1/2 nuclei under magic-angle spinning (MAS) conditions are investigated in detail.

The variable polarity plasma arc welding process: Characteristics and performance

Science.gov (United States)

Hung, R. J.; Zhu, G. J.

1991-01-01

Significant advantages of the Variable Polarity Plasma Arc (VPPA) Welding Process include faster welding, fewer repairs, less joint preparation, reduced weldment distortion, and absence of porosity. The power distribution was analyzed for an argon plasma gas flow constituting the fluid in the VPPA Welding Process. The major heat loss at the torch nozzle is convective heat transfer; in the space between the outlet of the nozzle and the workpiece; radiative heat transfer; and in the keyhole in the workpiece, convective heat transfer. The power absorbed at the workpiece produces the molten puddle that solidifies into the weld bead. Crown and root widths, and crown and root heights of the weld bead are predicted. The basis is provided for an algorithm for automatic control of VPPA welding machine parameters to obtain desired weld bead dimensions.

A Compendium of AGN inclinations with corresponding UV/optical continuum polarization measurements

Czech Academy of Sciences Publication Activity Database

Marin, Frederic

2014-01-01

Roč. 441, č. 1 (2014), s. 551-564 ISSN 0035-8711 Grant - others:ANR(FR) JS56-013-01; EU(XE) COST Action MP1104 Institutional support: RVO:67985815 Keywords : polarization * active galacticnuclei * radiative transfer Subject RIV: BN - Astronomy , Celestial Mechanics, Astrophysics Impact factor: 5.107, year: 2014

Electromagnetically induced absorption due to transfer of coherence and to transfer of population

International Nuclear Information System (INIS)

Goren, C.; Rosenbluh, M.; Wilson-Gordon, A.D.; Friedmann, H.

2003-01-01

The absorption spectrum of a weak probe, interacting with a driven degenerate two-level atomic system, whose ground and excited hyperfine states are F g,e , can exhibit narrow peaks at line center. When the pump and probe polarizations are different, F e =F g +1 and F g >0, the electromagnetically induced absorption (EIA) peak has been shown to be due to the transfer of coherence (TOC) between the excited and ground states via spontaneous decay. We give a detailed explanation of why the TOC that leads to EIA (EIA-TOC) can only take place when ground-state population trapping does not occur, that is, when F e =F g +1. We also explain why EIA-TOC is observed in open systems. We show that EIA can also occur when the pump and probe polarizations are identical and F e =F g +1. This EIA is analogous to an effect that occurs in simple two-level systems when the collisional transfer of population (TOP) from the ground state to a reservoir is greater than that from the excited state. For a degenerate two-level system, the reservoir consists of the Zeeman sublevels of the ground hyperfine state, and of other nearby hyperfine states that do not interact with the pump. We will also discuss the four-wave mixing spectrum under the conditions where EIA-TOC and EIA-TOP occur

Hydrogen exchange kinetics in a membrane protein determined by 15N NMR spectroscopy: Use of the INEPT [insensitive nucleus enhancement by polarization transfer] experiment to follow individual amides in detergent-solubilized M13 coat protein

International Nuclear Information System (INIS)

Henry, G.D.; Sykes, B.D.

1990-01-01

The coat protein of the filamentous coliphage M13 is a 50-residue polypeptide which spans the inner membrane of the Escherichia coli host upon infection. Amide hydrogen exchange kinetics have been used to probe the structure and dynamics of M13 coat protein which has been solubilized in sodium dodecyl sulfate (SDS) micelles. In a previous 1 H nuclear magnetic resonance (NMR) study, multiple exponential analysis of the unresolved amide proton envelope revealed the existence of two slow kinetic sets containing a total of about 30 protons. The slower set (15-20 amides) originates from the hydrophobic membrane-spanning region and exchanges at least 10 5 -fold slower than the unstructured, non-H-bonded model polypeptide poly(DL-alanine). Herein the authors use 15 N NMR spectroscopy of biosynthetically labeled coat protein to follow individual, assigned, slowly exchanging amides in or near the hydrophobic segment. The INEPT (insensitive nucleus enhancement by polarization transfer) experiments can be used to transfer magnetization to the 15 N nucleus from a coupled proton; when 15 N-labeled protonated protein is dissolved in 2 H 2 O, the INEPT signal disappears with time as the amide protons are replaced by solvent deuterons. Amide hydrogen exchange is catalyzed by both H + and OH - ions. The time-dependent exchange-out experiment is suitable for slow exchange rates (k ex ). The INEPT experiment was also adapted to measure some of the more rapidly exchanging amides in the coat protein using either saturation transfer from water or exchange effects on the polarization transfer step itself. The results of all of these experiments are consistent with previous models of the coat protein in which a stable segment extends from the hydrophobic membrane-spanning region through to the C-terminus, whereas the N-terminal region is undergoing more extensive dynamic fluctuations

Broadband non-polarizing beam splitter based on guided mode resonance effect

International Nuclear Information System (INIS)

Ma Jian-Yong; Xu Cheng; Qiang Ying-Huai; Zhu Ya-Bo

2011-01-01

A broadband non-polarizing beam splitter (NPBS) operating in the telecommunication C+L band is designed by using the guided mode resonance effect of periodic silicon-on-insulator (SOI) elements. It is shown that this double layer SOI structure can provide ∼50/50 beam ratio with the maximum divergences between reflection and transmission being less than 8% over the spectrum of 1.4 μm∼1.7 μm and 1% in the telecommunication band for both TE and TM polarizations. The physical basis of this broadband non-polarizing property is on the simultaneous excitation of the TE and TM strong modulation waveguide modes near the designed spectrum band. Meanwhile, the electric field distributions for both TE and TM polarizations verify the resonant origin of spectrum in the periodic SOI structure. Furthermore, it is demonstrated with our calculations that the beam splitter proposed here is tolerant to the deviations of incident angle and structure parameters, which make it very easy to be fabricated with current IC technology. (electromagnetism, optics, acoustics, heat transfer, classical mechanics, and fluid dynamics)

Conversion of proteins from a non-polarized to an apical secretory pattern in MDCK cells

International Nuclear Information System (INIS)

Vogel, Lotte K.; Larsen, Jakob E.; Hansen, Martin; Truffer, Renato

2005-01-01

Previously it was shown that fusion proteins containing the amino terminus of an apical targeted member of the serpin family fused to the corresponding carboxyl terminus of the non-polarized secreted serpin, antithrombin, are secreted mainly to the apical side of MDCK cells. The present study shows that this is neither due to the transfer of an apical sorting signal from the apically expressed proteins, since a sequence of random amino acids acts the same, nor is it due to the deletion of a conserved signal for correct targeting from the non-polarized secreted protein. Our results suggest that the polarity of secretion is determined by conformational sensitive sorting signals

Polarization memory of white luminescence of Ag nanoclusters dispersed in glass host.

Science.gov (United States)

Kuznetsov, A S; Tikhomirov, V K; Moshchalkov, V V

2012-09-10

A mechanism for white luminescence of Ag nanoclusters dispersed in oxyfluoride glass host has been revealed by studying a temperature dependence of its polarization memory. The spectral dependence of the polarization memory indicates the presence of a variety of Ag nanoclusters, particularly emitting in the blue, green and red. Temperature activated intercluster energy transfer has been found responsible for white luminescence. The means for increasing luminescence quantum yield have been suggested. This efficient white luminescence may be used in highly demanded devices, such as luminescent lamps, displays, color phosphors for LEDs, photovoltaic devices based on down shifting of solar spectrum.

3D Cloud Radiative Effects on Polarized Reflectances

Science.gov (United States)

Cornet, C.; Matar, C.; C-Labonnote, L.; Szczap, F.; Waquet, F.; Parol, F.; Riedi, J.

2017-12-01

As recognized in the last IPCC report, clouds have a major importance in the climate budget and need to be better characterized. Remote sensing observations are a way to obtain either global observations of cloud from satellites or a very fine description of clouds from airborne measurements. An increasing numbers of radiometers plan to measure polarized reflectances in addition to total reflectances, since this information is very helpful to obtain aerosol or cloud properties. In a near future, for example, the Multi-viewing, Multi-channel, Multi-polarization Imager (3MI) will be part the EPS-SG Eumetsat-ESA mission. It will achieve multi-angular polarimetric measurements from visible to shortwave infrared wavelengths. An airborne prototype, OSIRIS (Observing System Including Polarization in the Solar Infrared Spectrum), is also presently developed at the Laboratoire d'Optique Atmospherique and had already participated to several measurements campaigns. In order to analyze suitably the measured signal, it it necessary to have realistic and accurate models able to simulate polarized reflectances. The 3DCLOUD model (Szczap et al., 2014) was used to generate three-dimensional synthetic cloud and the 3D radiative transfer model, 3DMCPOL (Cornet et al., 2010) to compute realistic polarized reflectances. From these simulations, we investigate the effects of 3D cloud structures and heterogeneity on the polarized angular signature often used to retrieve cloud or aerosol properties. We show that 3D effects are weak for flat clouds but become quite significant for fractional clouds above ocean. The 3D effects are quite different according to the observation scale. For the airborne scale (few tens of meter), solar illumination effects can lead to polarized cloud reflectance values higher than the saturation limit predicted by the homogeneous cloud assumption. In the cloud gaps, corresponding to shadowed areas of the total reflectances, polarized signal can also be enhanced

Research on generating various polarization-modes in polarized illumination system

Science.gov (United States)

Huang, Jinping; Lin, Wumei; Fan, Zhenjie

2013-08-01

With the increase of the numerical aperture (NA), the polarization of light affects the imaging quality of projection lens more significantly. On the contrary, according to the mask pattern, the resolution of projection lens can be improved by using the polarized illumination. That is to say, using the corresponding polarized beam (or polarization-mode) along with the off-axis illumination will improve the resolution and the imaging quality of the of projection lens. Therefore, the research on the generation of various polarization modes and its conversion methods become more and more important. In order to realize various polarization modes in polarized illumination system, after read a lot of references, we provide a way that fitting for the illumination system with the wavelength of 193nm.Six polarization-modes and a depolarized mode are probably considered. Wave-plate stack is used to generate linearly polarization-mode, which have a higher degree polarization. In order to generate X-Y and Y-X polarization mode, the equipment consisting of four sectors of λ/2 wave plate was used. We combined 16 sectors of λ/2 wave plate which have different orientations of the "slow" axis to generate radial and azimuthal polarization. Finally, a multi-polarization control device was designed. Using the kind of multi-polarization control device which applying this method could help to choose the polarization modes conveniently and flexibility for the illumination system.

Polarization properties of linearly polarized parabolic scaling Bessel beams

Energy Technology Data Exchange (ETDEWEB)

Guo, Mengwen; Zhao, Daomu, E-mail: zhaodaomu@yahoo.com

2016-10-07

The intensity profiles for the dominant polarization, cross polarization, and longitudinal components of modified parabolic scaling Bessel beams with linear polarization are investigated theoretically. The transverse intensity distributions of the three electric components are intimately connected to the topological charge. In particular, the intensity patterns of the cross polarization and longitudinal components near the apodization plane reflect the sign of the topological charge. - Highlights: • We investigated the polarization properties of modified parabolic scaling Bessel beams with linear polarization. • We studied the evolution of transverse intensity profiles for the three components of these beams. • The intensity patterns of the cross polarization and longitudinal components can reflect the sign of the topological charge.

Study of kinetics and mechanism of diazo compound reactions using nuclear chemical polarization

International Nuclear Information System (INIS)

Gragerov, I.P.; Levit, A.F.; Kiprianova, L.A.; Buchachenko, A.L.; Sterleva, T.G.

1975-01-01

It has been established that at the rate-determining steps of the radical reactions in which aniline interacts with isoamyl nitrite and substituted diazo salts interact with sodium methylate, tertiary fatty amines, or phosphinic acid, no transfer of a single electron occurs. The processes of single electron transfer do not seem to play a decisive role in the kinetics of most transformations of diazo compounds. Chemical nuclear polarization is shown to be suitable for kinetic studies of fast radical processes

Transfer matrix approach for the Kerr and Faraday rotation in layered nanostructures

International Nuclear Information System (INIS)

Széchenyi, Gábor; Vigh, Máté; Cserti, József; Kormányos, Andor

2016-01-01

To study the optical rotation of the polarization of light incident on multilayer systems consisting of atomically thin conductors and dielectric multilayers we present a general method based on transfer matrices. The transfer matrix of the atomically thin conducting layer is obtained using the Maxwell equations. We derive expressions for the Kerr (Faraday) rotation angle and for the ellipticity of the reflected (transmitted) light as a function of the incident angle and polarization of the light. The method is demonstrated by calculating the Kerr (Faraday) angle for bilayer graphene in the quantum anomalous Hall state placed on the top of dielectric multilayers. The optical conductivity of the bilayer graphene is calculated in the framework of a four-band model. (paper)

Achieving highly efficient and broad-angle polarization beam filtering using epsilon-near-zero metamaterials mimicked by metal-dielectric multilayers

Science.gov (United States)

Wu, Feng

2018-03-01

We report a highly efficient and broad-angle polarization beam filter at visible wavelengths using an anisotropic epsilon-near-zero metamaterial mimicked by a multilayer composed of alternative subwavelength magnesium fluoride and silver layers. The underlying physics can be explained by the dramatic difference between two orthogonal polarizations' iso-frequency curves of anisotropic epsilon-near-zero metamaterials. Transmittance for two orthogonal polarization waves and the polarization extinction ratio are calculated via the transfer matrix method to assess the comprehensive performance of the proposed polarization beam filter. From the simulation results, the proposed polarization beam filter is highly efficient (the polarization extinction ratio is far larger than two orders of magnitude) and has a broad operating angle range (ranging from 30° to 75°). Finally, we show that the proper tailoring of the periodic number enables us to obtain high comprehensive performance of the proposed polarization beam filter.

Polarized nuclear target based on parahydrogen induced polarization

OpenAIRE

Budker, D.; Ledbetter, M. P.; Appelt, S.; Bouchard, L. S.; Wojtsekhowski, B.

2012-01-01

We discuss a novel concept of a polarized nuclear target for accelerator fixed-target scattering experiments, which is based on parahydrogen induced polarization (PHIP). One may be able to reach a 33% free-proton polarization in the ethane molecule. The potential advantages of such a target include operation at zero magnetic field, fast ($\\sim$100 Hz) polarization reversal, and operation with large intensity of an electron beam.

NMR of insensitive nuclei enhanced by dynamic nuclear polarization.

Science.gov (United States)

Miéville, Pascal; Jannin, Sami; Helm, Lothar; Bodenhausen, Geoffrey

2011-01-01

Despite the powerful spectroscopic information it provides, Nuclear Magnetic Resonance (NMR) spectroscopy suffers from a lack of sensitivity, especially when dealing with nuclei other than protons. Even though NMR can be applied in a straightforward manner when dealing with abundant protons of organic molecules, it is very challenging to address biomolecules in low concentration and/or many other nuclei of the periodic table that do not provide as intense signals as protons. Dynamic Nuclear Polarization (DNP) is an important technique that provides a way to dramatically increase signal intensities in NMR. It consists in transferring the very high electron spin polarization of paramagnetic centers (usually at low temperature) to the surrounding nuclear spins with appropriate microwave irradiation. DNP can lead to an enhancement of the nuclear spin polarization by up to four orders of magnitude. We present in this article some basic concepts of DNP, describe the DNP apparatus at EPFL, and illustrate the interest of the technique for chemical applications by reporting recent measurements of the kinetics of complexation of 89Y by the DOTAM ligand.

Calculation and construction of a beam-transport system for polarized electrons

International Nuclear Information System (INIS)

Marschke, G.

1987-09-01

In the framework of the ELSA-SAPHIR project a transfer channel between ELSA and the large-space detector SAPHIR was calculated and constructed. Existing optical elements were modified corresponding to their application and the missing racks constructed and ordered for fabrication. Furthermore the vacuum system was designed as the whole as well as in the single components. Starting from the architectonic conditions and the optics to be realized the coordinates of the elements were calculated as preconditions fo the geodetic measurements and calibrations. It was shown that both for a polarized and for an unpolarized electron beam an optic was realized corresponding to the requirements up to an energy of 3.5 GeV. Under the given conditions, the applied method of the rotation of the polarization vector, and the geometrical preconditions up to 3.0 GeV also an acceptable longitudinal polarization was reached. (orig./HSI) [de

Through space and through bridge channels of charge transfer at p-n nano-junctions: A DFT study

Energy Technology Data Exchange (ETDEWEB)

Dandu, Naveen [Department of Chemistry and Biochemistry, NDSU, Fargo, ND 58108 (United States); Tretiak, Sergei [Theoretical Division, Center for Nonlinear Studies (CNLS) and Center for Integrated Nanotechnologies (CINT), Los Alamos National Laboratory, Los Alamos, 57069, NM 87454 (United States); Kilina, Svetlana [Department of Chemistry and Biochemistry, NDSU, Fargo, ND 58108 (United States); Kilin, Dmitri, E-mail: Dmitri.Kilin@ndsu.edu [Department of Chemistry and Biochemistry, NDSU, Fargo, ND 58108 (United States)

2016-12-20

Highlights: • Properties of interacting QDs depend on the fashion of interaction: through-bond or through-space. • The disconnected and undoped dimer models shows FÓ§rster band formation. • Dimer models with some doping exhibit degenerate charge-transfer excitons. • p- and n-doped qds shows polarization at the interface. • A photoexcitation polarizes p-n interface, in relation to phototovoltaic effect. - Abstract: Details of charge density distribution at p-n nano interface are analyzed with density functional theory techniques using model system of dimers of doped silicon quantum dots interacting through bond and through space. Spatial distributions of transition densities between the ground and excited states suggest the character of essential electronic excitations, which have a FÓ§rster, bound, unbound, or charge transfer character. A redistribution of electronic density from n-impurities to p-impurities results in a ground state polarization and creates an offset of energies of the bands localized on p-doped quantum dot and the bands localized on n-doped quantum dot. Although impurities contribute very few orbitals to the total density, a ground state charge redistribution and polarization are both responsible for the presence of a large number of charge transfer excitations involving solely silicon orbitals.

THE HANLE AND ZEEMAN POLARIZATION SIGNALS OF THE SOLAR Ca II 8542 Å LINE

Energy Technology Data Exchange (ETDEWEB)

Štěpán, Jiri [Astronomical Institute ASCR, Fričova 298, 251 65 Ondřejov (Czech Republic); Bueno, Javier Trujillo [Instituto de Astrofísica de Canarias, E-38205 La Laguna, Tenerife (Spain)

2016-07-20

We highlight the main results of a three-dimensional (3D) multilevel radiative transfer investigation about the solar disk-center polarization of the Ca ii 8542 Å line. First, through the use of a 3D model of the solar atmosphere, we investigate the linear polarization that occurs due to the atomic level polarization produced by the absorption and scattering of anisotropic radiation, taking into account the symmetry-breaking effects caused by its thermal, dynamic, and magnetic structure. Second, we study the contribution of the Zeeman effect to the linear and circular polarization. Finally, we show examples of the Stokes profiles produced by the joint action of the atomic level polarization and the Hanle and Zeeman effects. We find that the Zeeman effect tends to dominate the linear polarization signals only in the localized patches of opposite magnetic polarity, where the magnetic field is relatively strong and slightly inclined; outside such very localized patches, the linear polarization is often dominated by the contribution of atomic level polarization. We demonstrate that a correct modeling of this last contribution requires taking into account the symmetry-breaking effects caused by the thermal, dynamic, and magnetic structure of the solar atmosphere, and that in the 3D model used the Hanle effect in forward-scattering geometry (disk-center observation) mainly reduces the polarization corresponding to the zero-field case. We emphasize that, in general, a reliable modeling of the linear polarization in the Ca ii 8542 Å line requires taking into account the joint action of atomic level polarization and the Hanle and Zeeman effects.

Fusion of a polarized projectile with a polarized target

International Nuclear Information System (INIS)

Christley, J.A.; Johnson, R.C.; Thompson, I.J.

1995-01-01

The fusion cross sections for a polarized target with both unpolarized and polarized projectiles are studied. Expressions for the observables are given for the case when both nuclei are polarized. Calculations for fusion of an aligned 165 Ho target with 16 O and polarized 7 Li beams are presented

Off-axis irradiation and the polarization of broad emission lines in active galactic nuclei

Czech Academy of Sciences Publication Activity Database

Goosmann, R. W.; Gaskell, C.M.; Marin, Frederic

2014-01-01

Roč. 54, č. 7 (2014), s. 1341-1346 ISSN 0273-1177 Institutional support: RVO:67985815 Keywords : polarization * radiative transfer * R line profiles Subject RIV: BN - Astronomy, Celestial Mechanics, Astrophysics OBOR OECD: Astronomy (including astrophysics,space science) Impact factor: 1.358, year: 2014

Study of xenon binding in cryptophane-A using laser-induced NMR polarization enhancement

International Nuclear Information System (INIS)

Luhmer, M.; Goodson, B.M.; Song, Y.Q.; Laws, D.D.; Kaiser, L.; Pines, A.; Lawrence Berkeley National Lab., CA

1999-01-01

Xenon is chemically inert, yet exhibits NMR parameters that are highly sensitive to its chemical environment. Considerable work has therefore capitalized on the utility of 129 Xe (I = 1/2) as a magnetic resonance probe of molecules, materials, and biological systems. In solution, spin-polarization transfer between laser-polarized xenon and the hydrogen nuclei of nearby molecules leads to signal enhancements in the resolved 1 H NMR spectrum, offering new opportunities for probing the chemical environment of xenon atoms. Following binding of laser-polarized xenon to molecules of cryptophane-A, selective enhancements of the 1 H NMR signals were observed. A theoretical framework for the interpretation of such experimental results is provided, and the spin polarization-induced nuclear Overhauser effects are shown to yield information about the molecular environment of xenon. The observed selective 1 H enhancements allowed xenon-proton internuclear distances to be estimated. These distances reveal structural characteristics of the complex, including the preferred molecular conformations adopted by cryptophane-A upon binding of xenon

Measurement of the average polarization of b baryons in hadronic $Z^0$ decays

CERN Document Server

Abbiendi, G.; Alexander, G.; Allison, John; Altekamp, N.; Anderson, K.J.; Anderson, S.; Arcelli, S.; Asai, S.; Ashby, S.F.; Axen, D.; Azuelos, G.; Ball, A.H.; Barberio, E.; Barlow, Roger J.; Bartoldus, R.; Batley, J.R.; Baumann, S.; Bechtluft, J.; Behnke, T.; Bell, Kenneth Watson; Bella, G.; Bellerive, A.; Bentvelsen, S.; Bethke, S.; Betts, S.; Biebel, O.; Biguzzi, A.; Bird, S.D.; Blobel, V.; Bloodworth, I.J.; Bobinski, M.; Bock, P.; Bohme, J.; Bonacorsi, D.; Boutemeur, M.; Braibant, S.; Bright-Thomas, P.; Brigliadori, L.; Brown, Robert M.; Burckhart, H.J.; Burgard, C.; Burgin, R.; Capiluppi, P.; Carnegie, R.K.; Carter, A.A.; Carter, J.R.; Chang, C.Y.; Charlton, David G.; Chrisman, D.; Ciocca, C.; Clarke, P.E.L.; Clay, E.; Cohen, I.; Conboy, J.E.; Cooke, O.C.; Couyoumtzelis, C.; Coxe, R.L.; Cuffiani, M.; Dado, S.; Dallavalle, G.Marco; Davis, R.; De Jong, S.; del Pozo, L.A.; De Roeck, A.; Desch, K.; Dienes, B.; Dixit, M.S.; Dubbert, J.; Duchovni, E.; Duckeck, G.; Duerdoth, I.P.; Eatough, D.; Estabrooks, P.G.; Etzion, E.; Evans, H.G.; Fabbri, F.; Fanti, M.; Faust, A.A.; Fiedler, F.; Fierro, M.; Fleck, I.; Folman, R.; Furtjes, A.; Futyan, D.I.; Gagnon, P.; Gary, J.W.; Gascon, J.; Gascon-Shotkin, S.M.; Gaycken, G.; Geich-Gimbel, C.; Giacomelli, G.; Giacomelli, P.; Gibson, V.; Gibson, W.R.; Gingrich, D.M.; Glenzinski, D.; Goldberg, J.; Gorn, W.; Grandi, C.; Gross, E.; Grunhaus, J.; Gruwe, M.; Hanson, G.G.; Hansroul, M.; Hapke, M.; Harder, K.; Hargrove, C.K.; Hartmann, C.; Hauschild, M.; Hawkes, C.M.; Hawkings, R.; Hemingway, R.J.; Herndon, M.; Herten, G.; Heuer, R.D.; Hildreth, M.D.; Hill, J.C.; Hillier, S.J.; Hobson, P.R.; Hocker, James Andrew; Homer, R.J.; Honma, A.K.; Horvath, D.; Hossain, K.R.; Howard, R.; Huntemeyer, P.; Igo-Kemenes, P.; Imrie, D.C.; Ishii, K.; Jacob, F.R.; Jawahery, A.; Jeremie, H.; Jimack, M.; Jones, C.R.; Jovanovic, P.; Junk, T.R.; Karlen, D.; Kartvelishvili, V.; Kawagoe, K.; Kawamoto, T.; Kayal, P.I.; Keeler, R.K.; Kellogg, R.G.; Kennedy, B.W.; Klier, A.; Kluth, S.; Kobayashi, T.; Kobel, M.; Koetke, D.S.; Kokott, T.P.; Kolrep, M.; Komamiya, S.; Kowalewski, Robert V.; Kress, T.; Krieger, P.; von Krogh, J.; Kuhl, T.; Kyberd, P.; Lafferty, G.D.; Lanske, D.; Lauber, J.; Lautenschlager, S.R.; Lawson, I.; Layter, J.G.; Lazic, D.; Lee, A.M.; Lellouch, D.; Letts, J.; Levinson, L.; Liebisch, R.; List, B.; Littlewood, C.; Lloyd, A.W.; Lloyd, S.L.; Loebinger, F.K.; Long, G.D.; Losty, M.J.; Ludwig, J.; Lui, D.; Macchiolo, A.; Macpherson, A.; Mader, W.; Mannelli, M.; Marcellini, S.; Markopoulos, C.; Martin, A.J.; Martin, J.P.; Martinez, G.; Mashimo, T.; Mattig, Peter; McDonald, W.John; McKenna, J.; Mckigney, E.A.; McMahon, T.J.; McPherson, R.A.; Meijers, F.; Menke, S.; Merritt, F.S.; Mes, H.; Meyer, J.; Michelini, A.; Mihara, S.; Mikenberg, G.; Miller, D.J.; Mir, R.; Mohr, W.; Montanari, A.; Mori, T.; Nagai, K.; Nakamura, I.; Neal, H.A.; Nellen, B.; Nisius, R.; O'Neale, S.W.; Oakham, F.G.; Odorici, F.; Ogren, H.O.; Oreglia, M.J.; Orito, S.; Palinkas, J.; Pasztor, G.; Pater, J.R.; Patrick, G.N.; Patt, J.; Perez-Ochoa, R.; Petzold, S.; Pfeifenschneider, P.; Pilcher, J.E.; Pinfold, J.; Plane, David E.; Poffenberger, P.; Polok, J.; Przybycien, M.; Rembser, C.; Rick, H.; Robertson, S.; Robins, S.A.; Rodning, N.; Roney, J.M.; Roscoe, K.; Rossi, A.M.; Rozen, Y.; Runge, K.; Runolfsson, O.; Rust, D.R.; Sachs, K.; Saeki, T.; Sahr, O.; Sang, W.M.; Sarkisian, E.K.G.; Sbarra, C.; Schaile, A.D.; Schaile, O.; Scharf, F.; Scharff-Hansen, P.; Schieck, J.; Schmitt, B.; Schmitt, S.; Schoning, A.; Schroder, Matthias; Schumacher, M.; Schwick, C.; Scott, W.G.; Seuster, R.; Shears, T.G.; Shen, B.C.; Shepherd-Themistocleous, C.H.; Sherwood, P.; Siroli, G.P.; Sittler, A.; Skuja, A.; Smith, A.M.; Snow, G.A.; Sobie, R.; Soldner-Rembold, S.; Sproston, M.; Stahl, A.; Stephens, K.; Steuerer, J.; Stoll, K.; Strom, David M.; Strohmer, R.; Surrow, B.; Talbot, S.D.; Tanaka, S.; Taras, P.; Tarem, S.; Teuscher, R.; Thiergen, M.; Thomson, M.A.; von Torne, E.; Torrence, E.; Towers, S.; Trigger, I.; Trocsanyi, Z.; Tsur, E.; Turcot, A.S.; Turner-Watson, M.F.; Van Kooten, Rick J.; Vannerem, P.; Verzocchi, M.; Voss, H.; Wackerle, F.; Wagner, A.; Ward, C.P.; Ward, D.R.; Watkins, P.M.; Watson, A.T.; Watson, N.K.; Wells, P.S.; Wermes, N.; White, J.S.; Wilson, G.W.; Wilson, J.A.; Wyatt, T.R.; Yamashita, S.; Yekutieli, G.; Zacek, V.; Zer-Zion, D.

1998-01-01

In the Standard Model, b quarks produced in e^+e^- annihilation at the Z^0 peak have a large average longitudinal polarization of -0.94. Some fraction of this polarization is expected to be transferred to b-flavored baryons during hadronization. The average longitudinal polarization of weakly decaying b baryons, , is measured in approximately 4.3 million hadronic Z^0 decays collected with the OPAL detector between 1990 and 1995 at LEP. Those b baryons that decay semileptonically and produce a \\Lambda baryon are identified through the correlation of the baryon number of the \\Lambda and the electric charge of the lepton. In this semileptonic decay, the ratio of the neutrino energy to the lepton energy is a sensitive polarization observable. The neutrino energy is estimated using missing energy measurements. From a fit to the distribution of this ratio, the value = -0.56^{+0.20}_{-0.13} +/- 0.09 is obtained, where the first error is statistical and the second systematic.

Influence of high range of mass transfer coefficient and convection heat transfer on direct contact membrane distillation performance

KAUST Repository

Lee, Jung Gil

2017-11-03

In order to improve water production of membrane distillation (MD), the development of high performance membrane having better mass transfer and enhancement of convection heat transfer in MD module have been continuously investigated. This paper presents the relationship between the heat and mass transfer resistance across the membrane and the performance improvement. Various ranges of mass transfer coefficient (MTC) from normal (0.3×10−6 to 2.1×10−6kg/m2sPa: currently available membranes) to high (>2.1×10−6kg/m2sPa: membranes under development) were simulated using an experimentally validated model at different ranges of convection heat transfer by varying the inlet flow rates and spacer enhancement factor. The effect of mass transfer and convection heat transfer on the MD performance parameters including temperature polarization coefficient (TPC), mean permeate flux, and specific energy consumption were investigated in a direct contact MD (DCMD) configuration. Results showed that improving the MTC at the low ranges is more important than that at the high ranges where the heat transfer resistance becomes dominant and hence the convection heat transfer coefficient must be increased. Therefore, an effort on designing MD modules using feed and permeate spacers and controlling the membrane surface roughness to increase the convection heat transfer and TPC in the channel aiming to enhance the flux is required because the currently developed mass transfer has almost reached the critical point.

Phase-transfer and film formation of silver nanoparticles.

Science.gov (United States)

Sarkar, Anjana; Chadha, Ridhima; Biswas, Nandita; Mukherjee, Tulsi; Kapoor, Sudhir

2009-04-01

In this article, a simple method for either transfer of silver nanoparticles from formamide to chloroform or to form a film at their interface is demonstrated. The transfer of the particles is a two-step size-dependent process. The size distribution of the colloidal hydrophobic silver particles in chloroform was almost the same as that before its transfer. Particles can be isolated by evaporation of chloroform. During evaporation, the hydrophobic particles become hydrophilic (charged) due to the formation of bilayer of CTAB over their surface. The isolated particles can be re-dispersed easily in polar solvents such as water and methanol. Nanocrystalline film of Ag is also prepared at the formamide-chloroform interface using suitable stabilizers in two immiscible layers. The nanocrystals have been characterized by various microscopic and spectroscopic techniques. The free standing film could be easily transferred on solid support.

Simulation of natural convection in an inclined polar cavity using a finite-difference lattice Boltzmann method

Energy Technology Data Exchange (ETDEWEB)

Yang, Fan; Yang, Haicheng; Guo, Xueyan; Ren Dai [University of Shanghai for Science and Technology, Shanghai (China); Yan, Yonghua [Shanghai Key Laboratory of Multiphase Flow and Heat Transfer in Power Engineering, Shanghai (China); Liu, Chaoqun [University of Texas at Arlington, Arlington (United States)

2017-06-15

Natural convection heat transfer in an inclined polar cavity was studied using a Finite-difference lattice Boltzmann method (FDLBM) based on a double-population approach for body-fitted coordinates. A D2G9 model coupled with the simplest TD2Q4 lattice model was applied to determine the velocity field and temperature field. For both velocity and temperature fields, the discrete spatial derivatives were obtained by combining the upwind scheme with the central scheme, and the discrete temporal term is obtained using a fourth-order Runge-Kutta scheme. Studies were carried out for different Rayleigh numbers and different inclination angles. The results in terms of streamlines, isotherms, and Nusselt numbers explain the heat transfer mechanism of natural convection in an inclined polar cavity due to the change of Rayleigh number and inclination angle.

Update of the Polar SWIFT model for polar stratospheric ozone loss (Polar SWIFT version 2)

Science.gov (United States)

Wohltmann, Ingo; Lehmann, Ralph; Rex, Markus

2017-07-01

The Polar SWIFT model is a fast scheme for calculating the chemistry of stratospheric ozone depletion in polar winter. It is intended for use in global climate models (GCMs) and Earth system models (ESMs) to enable the simulation of mutual interactions between the ozone layer and climate. To date, climate models often use prescribed ozone fields, since a full stratospheric chemistry scheme is computationally very expensive. Polar SWIFT is based on a set of coupled differential equations, which simulate the polar vortex-averaged mixing ratios of the key species involved in polar ozone depletion on a given vertical level. These species are O3, chemically active chlorine (ClOx), HCl, ClONO2 and HNO3. The only external input parameters that drive the model are the fraction of the polar vortex in sunlight and the fraction of the polar vortex below the temperatures necessary for the formation of polar stratospheric clouds. Here, we present an update of the Polar SWIFT model introducing several improvements over the original model formulation. In particular, the model is now trained on vortex-averaged reaction rates of the ATLAS Chemistry and Transport Model, which enables a detailed look at individual processes and an independent validation of the different parameterizations contained in the differential equations. The training of the original Polar SWIFT model was based on fitting complete model runs to satellite observations and did not allow for this. A revised formulation of the system of differential equations is developed, which closely fits vortex-averaged reaction rates from ATLAS that represent the main chemical processes influencing ozone. In addition, a parameterization for the HNO3 change by denitrification is included. The rates of change of the concentrations of the chemical species of the Polar SWIFT model are purely chemical rates of change in the new version, whereas in the original Polar SWIFT model, they included a transport effect caused by the

Measurement and calculation of polarization transfer coefficients in the reaction {sup 2}H(p,p){sup 2}H at E{sub p}=22.5 MeV

Energy Technology Data Exchange (ETDEWEB)

Clajus, M.; Albert, J.; Bruno, M.; Egun, P.M.; Glockle, W.; Glombik, A.; Gruebler, W.; Hautle, P.; Kretschmer, W.; Rauscher, A.; Schmelzbach, P.A.; Slaus, I.; Weidmann, R.; Witala, H. [Inst. fuer Mittelenergiephys., Eidgenoessische Tech. Hochschule, Zurich (Switzerland)

1995-10-01

The polarization transfer coefficients K{sub x}{sup x}', K{sub y}{sup y}' and K{sub z}{sup x}' in the reaction {sup 2}H(p,p){sup 2}H have been measured at an incident proton energy of 22.5 MeV. The results are compared to predictions from Faddeev calculations using various nucleon-nucleon potential models. The overall agreement is rather good. The comparison in more detail shows a pronounced sensitivity of the results, especially for K{sub y}{sup y}', to the {sup 3}S{sub 1}-{sup 3}D{sub 1} and {sup 1}P{sub 1} NN force components. As in nucleon-nucleon scattering, however, these two parameters are correlated, thus hampering definite conclusions. (author)

Radiative heat transfer between nanoparticles enhanced by intermediate particle

Directory of Open Access Journals (Sweden)

Yanhong Wang

2016-02-01

Full Text Available Radiative heat transfer between two polar nanostructures at different temperatures can be enhanced by resonant tunneling of surface polaritons. Here we show that the heat transfer between two nanoparticles is strongly varied by the interactions with a third nanoparticle. By controlling the size of the third particle, the time scale of thermalization toward the thermal bath temperature can be modified over 5 orders of magnitude. This effect provides control of temperature distribution in nanoparticle aggregation and facilitates thermal management at nanoscale.

{beta}-Carotene to bacteriochlorophyll c energy transfer in self-assembled aggregates mimicking chlorosomes

Energy Technology Data Exchange (ETDEWEB)

Alster, J. [Faculty of Mathematics and Physics, Charles University, Ke Karlovu 3, 121 16 Praha (Czech Republic); Polivka, T. [Institute of Physical Biology, University of South Bohemia, Zamek 136, 373 33 Nove Hrady (Czech Republic); Biology Centre, Academy of Sciences of the Czech Republic, Branisovska 31, 370 05 Ceske Budejovice (Czech Republic); Arellano, J.B. [Instituto de Recursos Naturales y Agrobiologia de Salamanca (IRNASA-CSIC), Apdo. 257, 37071 Salamanca (Spain); Chabera, P. [Institute of Physical Biology, University of South Bohemia, Zamek 136, 373 33 Nove Hrady (Czech Republic); Vacha, F. [Institute of Physical Biology, University of South Bohemia, Zamek 136, 373 33 Nove Hrady (Czech Republic); Biology Centre, Academy of Sciences of the Czech Republic, Branisovska 31, 370 05 Ceske Budejovice (Czech Republic); Psencik, J., E-mail: psencik@karlov.mff.cuni.cz [Faculty of Mathematics and Physics, Charles University, Ke Karlovu 3, 121 16 Praha (Czech Republic); Institute of Physical Biology, University of South Bohemia, Zamek 136, 373 33 Nove Hrady (Czech Republic)

2010-07-19

Carotenoids are together with bacteriochlorophylls important constituents of chlorosomes, the light-harvesting antennae of green photosynthetic bacteria. Majority of bacteriochlorophyll molecules form self-assembling aggregates inside the chlorosomes. Aggregates of bacteriochlorophylls with optical properties similar to those of chlorosomes can also be prepared in non-polar organic solvents or in aqueous environments when a suitable non-polar molecule is added. In this work, the ability of {beta}-carotene to induce aggregation of bacteriochlorophyll c in aqueous buffer was studied. Excitation relaxation and energy transfer in the carotenoid-bacteriochlorophyll assemblies were measured using femtosecond and nanosecond transient absorption spectroscopy. A fast, {approx}100-fs energy transfer from the S{sub 2} state of {beta}-carotene to bacteriochlorophyll c was revealed, while no evidence for significant energy transfer from the S{sub 1} state was found. Picosecond formation of the carotenoid triplet state (T{sub 1}) was observed, which was likely generated by singlet homo-fission from the S{sub 1} state of {beta}-carotene.

Spin transfer coefficient DΛLL to Λ hyperon in semi-inclusive DIS at HERMES

International Nuclear Information System (INIS)

Belostotski, S; Veretennikov, D; Naryshkin, Yu

2011-01-01

Three components of the spin transfer coefficient from the longitudinally polarized electron/positron beam to the Λ or Λ-bar hyperon have been measured in the HERMES experiment. Kinematical dependencies of the spin-transfer have been studied. Averaged over Λ kinematics, longitudinal component of the spin transfer DΛ LL (along the virtual photon direction) to the Λ hyperon is found to be DΛ LL = 0.19 ± 0.04 stat ± 0.02 syst .

Past, present and future polarization experiments with deuterons

International Nuclear Information System (INIS)

Punjabi, V.; Perdrisat, C.F.

1996-01-01

Recent experimental data for the inclusive breakup reaction A(d, p)X, with emphasis on 1 H(d, p)X, and the backward elastic scattering reaction dp → pd are discussed. There is now a fairly complete data base for these reactions, with measurements of the differential cross section, the tensor analyzing power T 20 and the deuteron to proton polarization transfer k 0 . The relevance of these reactions to the study of the short range properties of the deuteron is estimated [ru

Neutron polarization

International Nuclear Information System (INIS)

Firk, F.W.K.

1976-01-01

Some recent experiments involving polarized neutrons are discussed; they demonstrate how polarization studies provide information on fundamental aspects of nuclear structure that cannot be obtained from more traditional neutron studies. Until recently, neutron polarization studies tended to be limited either to very low energies or to restricted regions at higher energies, determined by the kinematics of favorable (p, vector n) and (d, vector n) reactions. With the advent of high intensity pulsed electron and proton accelerators and of beams of vector polarized deuterons, this is no longer the case. One has entered an era in which neutron polarization experiments are now being carried out, in a routine way, throughout the entire range from thermal energies to tens-of-MeV. The significance of neutron polarization studies is illustrated in discussions of a wide variety of experiments that include the measurement of T-invariance in the β-decay of polarized neutrons, a search for the effects of meson exchange currents in the photo-disintegration of the deuteron, the determination of quantum numbers of states in the fission of aligned 235 U and 237 Np induced by polarized neutrons, and the double- and triple-scattering of fast neutrons by light nuclei

Three-photon polarization ququarts: polarization, entanglement and Schmidt decompositions

International Nuclear Information System (INIS)

Fedorov, M V; Miklin, N I

2015-01-01

We consider polarization states of three photons, propagating collinearly and having equal given frequencies but with arbitrary distributed horizontal or vertical polarizations of photons. A general form of such states is a superposition of four basic three-photon polarization modes, to be referred to as the three-photon polarization ququarts (TPPQ). All such states can be considered as consisting of one- and two-photon parts, which can be entangled with each other. The degrees of entanglement and polarization, as well as the Schmidt decomposition and Stokes vectors of TPPQ are found and discussed. (paper)

Polarization splitter and polarization rotator designs based on transformation optics.

Science.gov (United States)

Kwon, Do-Hoon; Werner, Douglas H

2008-11-10

The transformation optics technique is employed in this paper to design two optical devices - a two-dimensional polarization splitter and a three-dimensional polarization rotator for propagating beams. The polarization splitter translates the TM- and the TE-polarized components of an incident beam in opposite directions (i.e., shifted up or shifted down). The polarization rotator rotates the polarization state of an incoming beam by an arbitrary angle. Both optical devices are reflectionless at the entry and exit interfaces. Design details and full-wave simulation results are provided.

Solar wind energy transfer regions inside the dayside magnetopause

International Nuclear Information System (INIS)

Lundin, R.; Dubinin, E.

1984-01-01

PROGNOZ-7 high temporal resolution measurements of the ion composition and hot plasma distribution in the dayside high latitude boundary layer near noon have revealed that magnetosheath plasma may penetrate the dayside magnetopause and form high density, high β, magnetosheath-like regions inside the magnetopause. From these measurements it is demonstrated that the magnetosheath injection regions most probably play an important role in transferring solar wind energy into the magnetosphere. The transfer regions are characterized by a strong perpendicular flow towards dawn or dusk (depending on local time) but are also observed to expand rapidly along the boundary field lines. This increased flow component transverse to the local magnetic field corresponds to a predominantly radial electric field of up to several mV m -1 , which indicates that the injected magnetosheath plasma causes an enhanced polarization of the boundary layer. Polarization of the boundary layer can therefore be considered a result of a local MHD-process where magnetosheath plasma excess momentum is converted into electromagnetic energy (electric field), i.e. there is an MHD-generator. It was observed that the boundary layer is charged up to tens of kilovolts, a potential which may be highly variable on e.g. the presence of a momentum exchange by the energy transfer regions. (author)

Polarization of recoil deuteron in ed elastic scattering at medium energies

International Nuclear Information System (INIS)

Bhalerao, R. S.

1981-12-01

Vector and tensor polarizations of the recoil deuteron in ed elastic scattering are calculated for THETA=0deg-180deg and q 2 2 . A longitudinally polarized electron beam is assumed to scatter off an unpolarized deuteron target. Calculations are made in the relativistic impulse approximation using a recently described approach based on the Bethe-Salpeter equation. Results are different, at high q 2 even qualitatively so, from those of a non-relativistic calculation, and a relativistic calculation which takes the spectator nucleon on-mass-shell. In the light of these results a recent suggestion that the polarization measurements would throw new light on the off-shell behavior and tensor force strength of the NN interaction are reexamined. Results are also presented for the three deuteron form factors Gsub(C), Gsub(Q), and Gsub(M), and the often-needed related quantities Ssub(S), Ssub(Q), and Ssub(M). The latter results may have an important implication in high-momentum transfer reactions involving deuteron. (author)

The Proton Coulomb Form Factor from Polarized Inclusive e-p Scattering

Energy Technology Data Exchange (ETDEWEB)

Harris, Christopher Matthew [Univ. of Virginia, Charlottesville, VA (United States)

2001-05-01

The proton form factors provide information on the fundamental properties of the proton and provide a test for models based on QCD. In 1998 at Jefferson Lab (JLAB) in Newport News, VA, experiment E93026 measured the inclusive e-p scattering cross section from a polarized ammonia (¹⁵NH₃) target at a four momentum transfer squared of Q² = 0.5 (GeV/c)². Longitudinally polarized electrons were scattered from the polarized target and the scattered electron was detected. Data has been analyzed to obtain the asymmetry from elastically scattered electrons from hydrogen in ¹⁵NH₃. The asymmetry, A_p, has been used to determine the proton elastic form factor G_Ep. The result is consistent with the dipole model and data from previous experiments. However, due to the choice of kinematics, the uncertainty in the measurement is large.

Dynamics of magnetization in ferromagnet with spin-transfer torque

Science.gov (United States)

Li, Zai-Dong; He, Peng-Bin; Liu, Wu-Ming

2014-11-01

We review our recent works on dynamics of magnetization in ferromagnet with spin-transfer torque. Driven by constant spin-polarized current, the spin-transfer torque counteracts both the precession driven by the effective field and the Gilbert damping term different from the common understanding. When the spin current exceeds the critical value, the conjunctive action of Gilbert damping and spin-transfer torque leads naturally the novel screw-pitch effect characterized by the temporal oscillation of domain wall velocity and width. Driven by space- and time-dependent spin-polarized current and magnetic field, we expatiate the formation of domain wall velocity in ferromagnetic nanowire. We discuss the properties of dynamic magnetic soliton in uniaxial anisotropic ferromagnetic nanowire driven by spin-transfer torque, and analyze the modulation instability and dark soliton on the spin wave background, which shows the characteristic breather behavior of the soliton as it propagates along the ferromagnetic nanowire. With stronger breather character, we get the novel magnetic rogue wave and clarify its formation mechanism. The generation of magnetic rogue wave mainly arises from the accumulation of energy and magnons toward to its central part. We also observe that the spin-polarized current can control the exchange rate of magnons between the envelope soliton and the background, and the critical current condition is obtained analytically. At last, we have theoretically investigated the current-excited and frequency-adjusted ferromagnetic resonance in magnetic trilayers. A particular case of the perpendicular analyzer reveals that the ferromagnetic resonance curves, including the resonant location and the resonant linewidth, can be adjusted by changing the pinned magnetization direction and the direct current. Under the control of the current and external magnetic field, several magnetic states, such as quasi-parallel and quasi-antiparallel stable states, out

Charge-Transfer States in Organic Solar Cells: Understanding the Impact of Polarization, Delocalization, and Disorder

KAUST Repository

Zheng, Zilong; Tummala, Naga Rajesh; Fu, Yao-Tsung; Coropceanu, Veaceslav; Bredas, Jean-Luc

2017-01-01

pentacene molecules and three C60 molecules allows us to take explicitly into account the electronic polarization effects. These complexes are extracted from a bilayer architecture modeled by molecular dynamics simulations and evaluated by means

Phospholipid transfer from vesicles to high density lipoproteins, catalyzed by human plasma phospholipid transfer protein

International Nuclear Information System (INIS)

Sweeny, S.A.

1985-01-01

Human plasma phospholipid transfer protein (PLTP) catalyzes the mass transfer of phosphatidylcholine (PC). Partial purification of PLTP yielded proteins with apparent M/sub r/ = 59,000 and 40,000 by SDS-PAGE. PLTP activity was measured by transfer of [ 14 C]L-α-dipalmitoyl PC from egg-PC vesicles to HDL. Activity was enhanced at low pH (4.5) upon addition of β-mercaptoethanol while Ca +2 and Na + had no effect. E/sub act/ for facilitated PC transfer was 18.2 +/- 2 kcal/mol. The donor specificity of PLTP was examined using vesicles containing egg-PC plus cholesterol or sphingomyelin. The fluidity of the donor membrane (measured by fluorescence polarization of diphenylhexatriene) correlated strongly with a decrease in PLTP activity. Phosphatidic acid did not affect activity. Increase in vesicle size reduced activity. The acceptor specificity of PLTP was examined using chemically modified HDL. PLTP activity increased up to 1.7-fold with an initial increase in negative charge and then decreased upon extensive modification. A mechanism is proposed where PLTP binds to vesicls and enhances the diffusion of PC into the medium where it is adsorbed by HDL

Development of the polarization tracking scheme for free-space quantum cryptography

Science.gov (United States)

Toyoshima, Morio; Takayama, Yoshihisa; Kunimori, Hiroo; Takeoka, Masahiro; Fujiwara, Mikio; Sasaki, Masahide

2008-04-01

Quantum cryptography is a new technique for transmitting quantum information. The information is securely transmitted due to the laws of physics. In such systems, the vehicle that transfers quantum information is a single photon. The problem with using photons is that the transmission distance is limited by the absorption of the photons by the optical fiber along which they pass. The maximum demonstrated range so far is approximately 100 km. Using free-space quantum cryptography between a ground station and a satellite is a possible way of sending quantum information farther than is possible with optical fibers. This is because there is no birefringence effect in the atmosphere. However, there is a complication in that the directions of the polarization basis between the transmitter and the receiver must coincide with each other. This polarization changes because the mobile terminals for free-space transmission continuously change their attitudes. If the transmission protocol is based on polarization, it is necessary to compensate for the change in attitude between the mobile terminals. We are developing a scheme to track the polarization basis between the transceivers. The preliminary result is presented.

Hair Mercury Concentrations in Western Hudson Bay Polar Bear Family Groups.

Science.gov (United States)

Bechshoft, Thea; Derocher, Andrew E; Richardson, Evan; Lunn, Nicholas J; St Louis, Vincent L

2016-05-17

Methylmercury is one of the more toxic forms of mercury (Hg), the biomagnification of which is prevalent in the Arctic where apex predators such as polar bears (Ursus maritimus) can carry high loads. The maternal transfer of contaminants to offspring is a concern, as offspring may be particularly sensitive to the effects of environmental pollutants during early development. However, few studies of polar bears report on Hg in dependent young. We examined hair total Hg (THg) concentrations in 24 polar bear family groups in western Hudson Bay: mother, cub-of-the-year (COY), yearling, and 2 year old. THg concentrations increased with bear age, with COYs having lower concentrations than other offspring groups (p ≤ 0.008). Using AICc-based regression models, we found maternal THg to be positively related to body condition and litter size, while overall offspring THg was positively related to maternal body condition in addition to being dependent on the sex and age of the offspring. COY THg concentrations were positively related to maternal THg while also depending on the sex of the offspring. Considering our results, future studies in polar bear ecotoxicology are encouraged to include offspring of different ages and sexes.

Polarization dynamics and polarization time of random three-dimensional electromagnetic fields

International Nuclear Information System (INIS)

Voipio, Timo; Setaelae, Tero; Shevchenko, Andriy; Friberg, Ari T.

2010-01-01

We investigate the polarization dynamics of random, stationary three-dimensional (3D) electromagnetic fields. For analyzing the time evolution of the instantaneous polarization state, two intensity-normalized polarization autocorrelation functions are introduced, one based on a geometric approach with the Poincare vectors and the other on energy considerations with the Jones vectors. Both approaches lead to the same conclusions on the rate and strength of the polarization dynamics and enable the definition of a polarization time over which the state of polarization remains essentially unchanged. For fields obeying Gaussian statistics, the two correlation functions are shown to be expressible in terms of quantities characterizing partial 3D polarization and electromagnetic coherence. The 3D degree of polarization is found to have the same meaning in the 3D polarization dynamics as the usual two-dimensional (2D) degree of polarization does with planar fields. The formalism is demonstrated with several examples, and it is expected to be useful in applications dealing with polarization fluctuations of 3D light.

Overview of polarization in intermediate energy nucleon-nucleus inelastic scattering

International Nuclear Information System (INIS)

Carey, T.

1985-01-01

The general role that polarization transfer (PT) can play in the ''dissection'' of medium-energy N-nucleus inelastic reactions is reviewed, specifically concentrating on the importance of complete sets of PT observables for the study of nuclear structure. The discussion is largely in the context of plane-wave impulse approximations, with the effects of distortions considered through comparisons between simple plane-wave predictions and DWIA computations. 31 refs., 11 figs

Polarized electron sources

Energy Technology Data Exchange (ETDEWEB)

Prepost, R. [Univ. of Wisconsin, Madison, WI (United States)

1994-12-01

The fundamentals of polarized electron sources are described with particular application to the Stanford Linear Accelerator Center. The SLAC polarized electron source is based on the principle of polarized photoemission from Gallium Arsenide. Recent developments using epitaxially grown, strained Gallium Arsenide cathodes have made it possible to obtain electron polarization significantly in excess of the conventional 50% polarization limit. The basic principles for Gallium and Arsenide polarized photoemitters are reviewed, and the extension of the basic technique to strained cathode structures is described. Results from laboratory measurements of strained photocathodes as well as operational results from the SLAC polarized source are presented.

Polarized electron sources

International Nuclear Information System (INIS)

Prepost, R.

1994-01-01

The fundamentals of polarized electron sources are described with particular application to the Stanford Linear Accelerator Center. The SLAC polarized electron source is based on the principle of polarized photoemission from Gallium Arsenide. Recent developments using epitaxially grown, strained Gallium Arsenide cathodes have made it possible to obtain electron polarization significantly in excess of the conventional 50% polarization limit. The basic principles for Gallium and Arsenide polarized photoemitters are reviewed, and the extension of the basic technique to strained cathode structures is described. Results from laboratory measurements of strained photocathodes as well as operational results from the SLAC polarized source are presented

X-ray polarization fluctuations induced by cloud eclipses in active galactic nuclei

Czech Academy of Sciences Publication Activity Database

Marin, Frederic; Dovčiak, Michal

2015-01-01

Roč. 573, January (2015), A60/1-A60/8 ISSN 0004-6361 R&D Projects: GA MŠk LD12010 Grant - others:EU(XE) COST action MP1104 Institutional support: RVO:67985815 Keywords : galaxies: Seyfert * polarization * radiative transfer * relativistic processes * scattering * X-rays: general Subject RIV: BN - Astronomy, Celestial Mechanics, Astrophysics Impact factor: 4.378, year: 2014

Update of the Polar SWIFT model for polar stratospheric ozone loss (Polar SWIFT version 2

Directory of Open Access Journals (Sweden)

I. Wohltmann

2017-07-01

Full Text Available The Polar SWIFT model is a fast scheme for calculating the chemistry of stratospheric ozone depletion in polar winter. It is intended for use in global climate models (GCMs and Earth system models (ESMs to enable the simulation of mutual interactions between the ozone layer and climate. To date, climate models often use prescribed ozone fields, since a full stratospheric chemistry scheme is computationally very expensive. Polar SWIFT is based on a set of coupled differential equations, which simulate the polar vortex-averaged mixing ratios of the key species involved in polar ozone depletion on a given vertical level. These species are O3, chemically active chlorine (ClOx, HCl, ClONO2 and HNO3. The only external input parameters that drive the model are the fraction of the polar vortex in sunlight and the fraction of the polar vortex below the temperatures necessary for the formation of polar stratospheric clouds. Here, we present an update of the Polar SWIFT model introducing several improvements over the original model formulation. In particular, the model is now trained on vortex-averaged reaction rates of the ATLAS Chemistry and Transport Model, which enables a detailed look at individual processes and an independent validation of the different parameterizations contained in the differential equations. The training of the original Polar SWIFT model was based on fitting complete model runs to satellite observations and did not allow for this. A revised formulation of the system of differential equations is developed, which closely fits vortex-averaged reaction rates from ATLAS that represent the main chemical processes influencing ozone. In addition, a parameterization for the HNO3 change by denitrification is included. The rates of change of the concentrations of the chemical species of the Polar SWIFT model are purely chemical rates of change in the new version, whereas in the original Polar SWIFT model, they included a transport effect

Experimental and theoretical analyses of temperature polarization effect in vacuum membrane distillation

KAUST Repository

Alsaadi, Ahmad Salem; Francis, Lijo; Amy, Gary L.; Ghaffour, NorEddine

2014-01-01

This paper discusses the effect of temperature polarization in Vacuum Membrane Distillation (VMD). The main motivation for using VMD in this work is that this module configuration is much simpler and more suitable for this kind of investigation than the other MD configurations such as Direct Contact Membrane Distillation (DCMD). The coupling between heat and mass transfer mechanisms at the feed-membrane interface is presented from a theoretical point of view. In addition, a new simple graphical method and a mathematical model for determining VMD flux are presented. The two methods used in evaluating the extent of temperature polarization effect on water vapor flux (flux sensitivity factors and temperature polarization coefficient (TPC)) are also analyzed and compared. The effect of integrating a heat recovery system in a large scale module on the TPC coefficient has also been studied and presented in this paper. © 2014 Elsevier B.V.

Experimental and theoretical analyses of temperature polarization effect in vacuum membrane distillation

KAUST Repository

Alsaadi, Ahmad Salem

2014-08-13

This paper discusses the effect of temperature polarization in Vacuum Membrane Distillation (VMD). The main motivation for using VMD in this work is that this module configuration is much simpler and more suitable for this kind of investigation than the other MD configurations such as Direct Contact Membrane Distillation (DCMD). The coupling between heat and mass transfer mechanisms at the feed-membrane interface is presented from a theoretical point of view. In addition, a new simple graphical method and a mathematical model for determining VMD flux are presented. The two methods used in evaluating the extent of temperature polarization effect on water vapor flux (flux sensitivity factors and temperature polarization coefficient (TPC)) are also analyzed and compared. The effect of integrating a heat recovery system in a large scale module on the TPC coefficient has also been studied and presented in this paper. © 2014 Elsevier B.V.

Polar surface energies of iono-covalent materials: implications of a charge-transfer model tested on Li2FeSiO4 surfaces.

Science.gov (United States)

Hörmann, Nicolas G; Groß, Axel

2014-07-21

The ionic compounds that are used as electrode materials in Li-based rechargeable batteries can exhibit polar surfaces that in general have high surface energies. We derive an analytical estimate for the surface energy of such polar surfaces assuming charge redistribution as a polarity compensating mechanism. The polar contribution to the converged surface energy is found to be proportional to the bandgap multiplied by the surface charge necessary to compensate for the depolarization field, and some higher order correction terms that depend on the specific surface. Other features, such as convergence behavior, coincide with published results. General conclusions are drawn on how to perform polar surface energy calculations in a slab configuration and upper boundaries of "purely" polar surface energies are estimated. Furthermore, we compare these findings with results obtained in a density functional theory study of Li(2)FeSiO(4) surfaces. We show that typical polar features are observed and provide a decomposition of surface energies into polar and local bond-cutting contributions for 29 different surfaces. We show that the model is able to explain subtle differences of GGA and GGA+U surface energy calculations. © 2014 WILEY-VCH Verlag GmbH & Co. KGaA, Weinheim.

Mathematical and numerical analysis of systems of compressible hydrodynamics and photonics with polar coordinates

International Nuclear Information System (INIS)

Meltz, Bertrand

2015-01-01

This thesis deals with the mathematical and numerical analysis of the systems of compressible hydrodynamics and radiative transfer. More precisely, we study the derivation of numerical methods with 2D polar coordinates (one for the radius, one for the angle) where equations are discretized on regular polar grids. On one hand, these methods are well-suited for the simulation of flows with polar symmetries since they preserve these symmetries by construction. On the other hand, such coordinates systems introduce geometrical singularities as well as geometrical source terms which must be carefully treated. The first part of this document is devoted to the study of hydrodynamics equations, or Euler equations. We propose a new class of arbitrary high-order numerical schemes in both space and time and rely on directional splitting methods for the resolution of 2D equations. Each sub-system is solved using a Lagrange+Remap solver. We study the influence of the r=0 geometrical singularities of the cylindrical and spherical coordinates systems on the precision of the 2D numerical solutions. The second part of this document is devoted to the study of radiative transfer equations. In these equations, the unknowns depend on a large number of variables and a stiff source term is involved. The main difficulty consists in capturing the correct asymptotic behavior on coarse grids. We first construct a class of models where the radiative intensity is projected on a truncated spherical harmonics basis in order to lower the number of mathematical dimensions. Then we propose an Asymptotic Preserving scheme built in polar coordinates and we show that the scheme capture the correct diffusion limit in the radial direction as well as in the polar direction. (author) [fr

Promoting Diversity Through Polar Interdisciplinary Coordinated Education (Polar ICE)

Science.gov (United States)

McDonnell, J. D.; Hotaling, L. A.; Garza, C.; Van Dyk, P. B.; Hunter-thomson, K. I.; Middendorf, J.; Daniel, A.; Matsumoto, G. I.; Schofield, O.

2017-12-01

Polar Interdisciplinary Coordinated Education (ICE) is an education and outreach program designed to provide public access to the Antarctic and Arctic regions through polar data and interactions with the scientists. The program provides multi-faceted science communication training for early career scientists that consist of a face-to face workshop and opportunities to apply these skills. The key components of the scientist training workshop include cultural competency training, deconstructing/decoding science for non-expert audiences, the art of telling science stories, and networking with members of the education and outreach community and reflecting on communication skills. Scientists partner with educators to provide professional development for K-12 educators and support for student research symposia. Polar ICE has initiated a Polar Literacy initiative that provides both a grounding in big ideas in polar science and science communication training designed to underscore the importance of the Polar Regions to the public while promoting interdisciplinary collaborations between scientists and educators. Our ultimate objective is to promote STEM identity through professional development of scientists and educators while developing career awareness of STEM pathways in Polar science.

Polarization-independent broadband meta-holograms via polarization-dependent nanoholes.

Science.gov (United States)

Zhang, Xiaohu; Li, Xiong; Jin, Jinjin; Pu, Mingbo; Ma, Xiaoliang; Luo, Jun; Guo, Yinghui; Wang, Changtao; Luo, Xiangang

2018-05-17

Composed of ultrathin metal or dielectric nanostructures, metasurfaces can manipulate the phase, amplitude and polarization of electromagnetic waves at a subwavelength scale, which is promising for flat optical devices. In general, metasurfaces composed of space-variant anisotropic units are sensitive to the incident polarization due to the inherent polarization dependent geometric phase. Here, we implement polarization-independent broadband metasurface holograms constructed by polarization-dependent anisotropic elliptical nanoholes by elaborate design of complex amplitude holograms. The fabricated meta-hologram exhibits a polarization insensitive feature with an acceptable image quality. We verify the feasibility of the design algorithm for three-dimensional (3D) meta-holograms with simulation and the feasibility for two-dimensional (2D) meta-holograms is experimentally demonstrated at a broadband wavelength range from 405 nm to 632.8 nm. The effective polarization-independent broadband complex wavefront control with anisotropic elliptical nanoholes proposed in this paper greatly promotes the practical applications of the metasurface in technologies associated with wavefront manipulation, such as flat lens, colorful holographic displays and optical storage.

Non-catalytic transfer hydrogenation in supercritical CO2 for coal liquefaction

Science.gov (United States)

Elhussien, Hussien

This thesis presents the results of the investigation on developing and evaluating a low temperature (coal dissolution in supercritical CO2. The main idea behind the thesis was that one hydrogen atom from water and one hydrogen atom from the hydrogen transfer agent (HTA) were used to hydrogenate the coal. The products of coal dissolution were non-polar and polar while the supercritical CO2, which enhanced the rates of hydrogenation and dissolution of the non-polar molecules and removal from the reaction site, was non-polar. The polar modifier (PM) for CO2 was added to the freed to aid in the dissolution and removal of the polar components. The addition of a phase transfer agent (PTA) allowed a seamless transport of the ions and by-product between the aqueous and organic phases. DDAB, used as the PTA, is an effective phase transfer catalyst and showed enhancement to the coal dissolution process. COAL + DH- +H 2O → COAL.H2 + DHO-- This process has a great feature due to the fact that the chemicals were obtained without requir-ing to first convert coal to CO and H2 units as in indirect coal liquefaction. The experiments were conducted in a unique reactor set up that can be connected through two lines. one line to feed the reactor with supercritical CO 2 and the other connected to gas chromatograph. The use of the supercritical CO2 enhanced the solvent option due to the chemical extraction, in addition to the low environmental impact and energy cost. In this thesis the experiment were conducted at five different temperatures from atmos-pheric to 140°C, 3000 - 6000 psi with five component of feed mixture, namely water, HTA, PTA, coal, and PM in semi batch vessels reactor system with a volume of 100 mL. The results show that the chemicals were obtained without requiring to first convert coal to CO and H2 units as in indirect coal liquefaction. The results show that the conversion was found to be 91.8% at opti-mum feed mixtures values of 3, 1.0 and 5.4 for water: PM

Spin waves in full-polarized state of Dzyaloshinskii-Moriya helimagnets: Small-angle neutron scattering study

Science.gov (United States)

Grigoriev, S. V.; Sukhanov, A. S.; Altynbaev, E. V.; Siegfried, S.-A.; Heinemann, A.; Kizhe, P.; Maleyev, S. V.

2015-12-01

We develop the technique to study the spin-wave dynamics of the full-polarized state of the Dzyaloshinskii-Moriya helimagnets by polarized small-angle neutron scattering. We have experimentally proven that the spin-waves dispersion in this state has the anisotropic form. We show that the neutron scattering image displays a circle with a certain radius which is centered at the momentum transfer corresponding to the helix wave vector in helimagnetic phase ks, which is oriented along the applied magnetic field H . The radius of this circle is directly related to the spin-wave stiffness of this system. This scattering depends on the neutron polarization showing the one-handed nature of the spin waves in Dzyaloshinskii-Moriya helimagnets in the full-polarized phase. We show that the spin-wave stiffness A for MnSi helimagnet decreased twice as the temperature increases from zero to the critical temperature Tc.

Polarization digital holographic microscopy using low-cost liquid crystal polarization rotators

Science.gov (United States)

Dovhaliuk, Rostyslav Yu

2018-02-01

Polarization imaging methods are actively used to study anisotropic objects. A number of methods and systems, such as imaging polarimeters, were proposed to measure the state of polarization of light that passed through the object. Digital holographic and interferometric approaches can be used to quantitatively measure both amplitude and phase of a wavefront. Using polarization modulation optics, the measurement capabilities of such interference-based systems can be extended to measure polarization-dependent parameters, such as phase retardation. Different kinds of polarization rotators can be used to alternate the polarization of a reference beam. Liquid crystals are used in a rapidly increasing number of different optoelectronic devices. Twisted nematic liquid crystals are widely used as amplitude modulators in electronic displays and light valves or shutter glass. Such devices are of particular interest for polarization imaging, as they can be used as polarization rotators, and due to large-scale manufacturing have relatively low cost. A simple Mach-Zehnder polarized holographic setup that uses modified shutter glass as a polarization rotator is demonstrated. The suggested approach is experimentally validated by measuring retardation of quarter-wave film.

Measuring absolute spin polarization in dissolution-DNP by Spin PolarimetrY Magnetic Resonance (SPY-MR).

OpenAIRE

Vuichoud , Basile; Milani , Jonas; Chappuis , Quentin; Bornet , Aurélien; Bodenhausen , Geoffrey; Jannin , Sami

2015-01-01

Dynamic nuclear polarization at 1.2 K and 6.7 T allows one to achieve spin temperatures on the order of a few millikelvin, so that the high-temperature approximation (Delta E < kT) is violated for the nuclear Zeeman interaction Delta E = gamma B(0)h/(2 pi) of most isotopes. Provided that, after rapid dissolution and transfer to an NMR or MRI system, the hyperpolarized molecules contain at least two nuclear spins I and S with a scalar coupling J(IS), the polarization of spin I (short for 'inve...

A new instrumental set-up for polarized neutron scattering experiments

International Nuclear Information System (INIS)

Schmidt, Wolfgang; Ohl, Michael

2005-01-01

Neutron scattering with polarization analysis is a powerful tool to determine magnetic structures and excitations. A common setup is to mount the sample at the center of a Helmholtz-type coil which can provide a magnetic field of any direction at the sample position and also a guide field along the neutron flight paths around the sample. Recent experiments showed quite a high demand for measurements at low momentum transfers. For the corresponding low scattering angles air scattering gives rise to a very large background. For this reason we have extended the standard setup to a combination of a large vacuum tank surrounded by electrical coils. The vacuum tank eliminates the air scattering and we can use the polarization analysis down to the lowest accessible momentum transfers. The coils themselves also show some new features: In contrary to the classic (symmetric) coil distribution we use an asymmetric setup which gives the advantage of a larger scattering window. Due to a more sophisticated current distribution this modified coil arrangement needs not to be rotated for different scattering conditions. The whole set-up will soon be available at IN12, a cold neutrons three-axis spectrometer operated by FZ Juelich in collaboration with CEA Grenoble as a CRG-B instrument at the Institut Laue Langevin in Grenoble

Solvent polarity scale on the fluorescence spectra of a dansyl monomer copolymerizable in aqueous media

Science.gov (United States)

Ren, Biye; Gao, Feng; Tong, Zhen; Yan, Yu

1999-06-01

A copolymerizable fluorescent monomer N-[2-[[[5-(N,N-dimethylamino)-1-naphthalenyl]sulfonyl]-amino]ethyl]-2-propenamide (DANSAEP) was synthesized, which exhibits dual fluorescence due to the twisted intramolecular charge transfer in the excited state. The emission maximum λem shifts from 463.3 nm in n-hexane to 530.0 nm in water, showing solvent polarity dependence. The relations between λem and the conventional solvent polarity parameters ET(30) or Z are linear, dividing solvents into protic and aprotic groups. Kamlet's linear solvation energy relationship gives a good description for λem as a solvent polarity scale. The increment of dipole moment Δ μ at the excited state was estimated as 5.09 D with the solvatochromic analysis.

A Polarizable and Transferable PHAST CO 2 Potential for Materials Simulation

KAUST Repository

Mullen, Ashley L.

2013-12-10

Reliable PHAST (Potentials with High Accuracy Speed and Transferability) intermolecular potential energy functions for CO2 have been developed from first principles for use in heterogeneous systems, including one with explicit polarization. The intermolecular potentials have been expressed in a transferable form and parametrized from nearly exact electronic structure calculations. Models with and without explicit many-body polarization effects, known to be important in simulation of interfacial processes, are constructed. The models have been validated on pressure-density isotherms of bulk CO 2 and adsorption in three metal-organic framework (MOF) materials. The present models appear to offer advantages over high quality fluid/liquid state potentials in describing CO2 interactions in interfacial environments where sorbates adopt orientations not commonly explored in bulk fluids. Thus, the nonpolar CO2-PHAST and polarizable CO 2-PHAST* potentials are recommended for materials/interfacial simulations. © 2013 American Chemical Society.

The Mars water cycle at other epochs - Recent history of the polar caps and layered terrain

Science.gov (United States)

Jakosky, Bruce M.; Henderson, Bradley G.; Mellon, Michael T.

1993-01-01

A numerical model is presented of the integrated role of seasonal water cycle on the evolution of polar deposits on Mars over the last 10 million years. From the model, it is concluded that the only major difference between the polar caps which affects their long-term behavior is ultimately the difference in their elevations. Because of that difference, there is a preference for CO2 frost to stay longer on the northern polar cap. The average difference in sublimation at the caps results in a net south-to-north transport of water ice over long time scales. Superimposed on any long-term behavior is a transfer of water ice between the caps on the 10 exp 5 - 10 exp 6 yr time scales. The amount of water exchanged is small compared to the total ice content of the polar deposits.

Photodegradation and polarization properties of vertical external surface-emitting organic laser

International Nuclear Information System (INIS)

Leang, Tatiana

2014-01-01

Although organic solid-state dye lasers can provide wavelength tunability in the whole visible spectrum and offers perspectives of low-cost compact lasers, they are still limited by several drawbacks, especially photodegradation. The geometry of a Vertical External Cavity Surface-emitting Organic Laser (VECSOL) enables organic lasers to reach high energies, excellent conversion efficiencies and good beam quality, it also enables an external control on many parameters, a feature that we have used here to study the photodegradation phenomenon as well as some polarization properties of organic solid-state lasers. In the first part of this thesis, we studied the lifetime of the laser upon varying several parameters (pump pulse-width, repetition rate, output coupling,...) and we found that the intracavity laser intensity, independently of the pump intensity, had a major on photodegradation rate. Moreover, we observed that the profile of the laser beam was also degrading with time: while it is Gaussian in the beginning it gradually shifts to an annular shape. In the second part, we investigated the polarization properties of VECSOLs, with a special emphasis on fluorescence properties of some typical dyes used in lasers. The crucial role played by resonant non-radiative energy transfers between dye molecules (HOMO-FRET) is evidenced and enables explaining the observed fluorescence depolarization, compared to the expected limiting fluorescence anisotropy. Energy transfers happen to play a negligible role above laser threshold, as the organic laser beam is shown to be linearly polarized in a wide range of experimental conditions when excitation occurs in the first singlet state. (author) [fr

d-PET-controlled “off-on” Polarity-sensitive Probes for Reporting Local Hydrophilicity within Lysosomes

Science.gov (United States)

Zhu, Hao; Fan, Jiangli; Mu, Huiying; Zhu, Tao; Zhang, Zhen; Du, Jianjun; Peng, Xiaojun

2016-10-01

Polarity-sensitive fluorescent probes are powerful chemical tools for studying biomolecular structures and activities both in vitro and in vivo. However, the lack of “off-on” polarity-sensing probes has limited the accurate monitoring of biological processes that involve an increase in local hydrophilicity. Here, we design and synthesize a series of “off-on” polarity-sensitive fluorescent probes BP series consisting of the difluoroboron dippyomethene (BODIPY) fluorophore connected to a quaternary ammonium moiety via different carbon linkers. All these probes showed low fluorescence quantum yields in nonpolar solution but became highly fluorescent in polar media. BP-2, which contains a two-carbon linker and a trimethyl quaternary ammonium, displayed a fluorescence intensity and quantum yield that were both linearly correlated with solvent polarity. In addition, BP-2 exhibited high sensitivity and selectivity for polarity over other environmental factors and a variety of biologically relevant species. BP-2 can be synthesized readily via an unusual Mannich reaction followed by methylation. Using electrochemistry combined with theoretical calculations, we demonstrated that the “off-on” sensing behavior of BP-2 is primarily due to the polarity-dependent donor-excited photoinduced electron transfer (d-PET) effect. Live-cell imaging established that BP-2 enables the detection of local hydrophilicity within lysosomes under conditions of lysosomal dysfunction.

Low-Temperature Dynamic Nuclear Polarization at 9.4 Tesla With a 30 Milliwatt Microwave Source

Science.gov (United States)

Thurber, Kent R.; Yau, Wai-Ming; Tycko, Robert

2010-01-01

Dynamic nuclear polarization (DNP) can provide large signal enhancements in nuclear magnetic resonance (NMR) by transfer of polarization from electron spins to nuclear spins. We discuss several aspects of DNP experiments at 9.4 Tesla (400 MHz resonant frequency for 1H, 264 GHz for electron spins in organic radicals) in the 7–80 K temperature range, using a 30 mW, frequency-tunable microwave source and a quasi-optical microwave bridge for polarization control and low-loss microwave transmission. In experiments on frozen glycerol/water doped with nitroxide radicals, DNP signal enhancements up to a factor of 80 are observed (relative to 1H NMR signals with thermal equilibrium spin polarization). The largest sensitivity enhancements are observed with a new triradical dopant, DOTOPA-TEMPO. Field modulation with a 10 G root-mean-squared amplitude during DNP increases the nuclear spin polarizations by up to 135%. Dependencies of 1H NMR signal amplitudes, nuclear spin relaxation times, and DNP build-up times on the dopant and its concentration, temperature, microwave power, and modulation frequency are reported and discussed. The benefits of low-temperature DNP can be dramatic: the 1H spin polarization is increased approximately 1000-fold at 7 K with DNP, relative to thermal polarization at 80 K. PMID:20392658

Contribution of parsec-scale material onto the polarized X-ray spectrum of type-1 Seyfert galaxies

Science.gov (United States)

Marin, F.; Dovčiak, M.; Kammoun, E. S.

2018-04-01

Type-1 radio-quiet active galactic nuclei (AGN) are seen from the polar direction and offer a direct view of their central X-ray engine. If most of X-ray photons have traveled from the primary source to the observer with minimum light-matter interaction, a fraction of radiation is emitted at different directions and is reprocessed by the parsec-scale equatorial circumnuclear region or the polar outflows. It is still unclear how much the polarization expected from type-1 AGN is affected by radiation that have scattered on the distant AGN components. In this paper, we examine the contribution of remote material onto the polarized X-ray spectrum of type-1 Seyfert galaxies using radiative transfer Monte Carlo codes. We find that the observed X-ray polarization strongly depends on the initial polarization emerging from the disk-corona system. For unpolarized and parallelly polarized photons (parallel to the disk), the contribution is negligible below 3 keV and tends to increase the polarization degree by up to one percentage points at higher energies, smoothing out the energy-dependent variations of the polarization angle. For perpendicularly polarized corona photons, the addition of the circumnuclear scattered (parallel) component adds to the polarization above 10keV, decreases polarization below 10 keV and shifts the expected 90° rotation of the polarization angle to lower energies. In conclusion, we found that simulations of Seyfert-1s that do not account for reprocessing on the parsec-scale equatorial and polar material are under- or over-estimating the X-ray polarization by 0.1 - 1 percentage points.

IGS polar motion measurement accuracy

Directory of Open Access Journals (Sweden)

Jim Ray

2017-11-01

Full Text Available We elaborate an error budget for the long-term accuracy of IGS (International Global Navigation Satellite System Service polar motion estimates, concluding that it is probably about 25–30 μas (1-sigma overall, although it is not possible to quantify possible contributions (mainly annual that might transfer directly from aliases of subdaily rotational tide errors. The leading sources are biases arising from the need to align daily, observed terrestrial frames, within which the pole coordinates are expressed and which are continuously deforming, to the secular, linear international reference frame. Such biases are largest over spans longer than about a year. Thanks to the very large number of IGS tracking stations, the formal covariance errors are much smaller, around 5 to 10 μas. Large networks also permit the systematic frame-related errors to be more effectively minimized but not eliminated. A number of periodic errors probably also influence polar motion results, mainly at annual, GPS (Global Positioning System draconitic, and fortnightly periods, but their impact on the overall error budget is unlikely to be significant except possibly for annual tidal aliases. Nevertheless, caution should be exercised in interpreting geophysical excitations near any of the suspect periods.

Control letters and uncertainties of the kerma patterns in air, dose absorbed in water and dose absorbed in air of the LSCD; Cartas de control e incertidumbres de los patrones de kerma en aire, dosis absorbida en agua y dosis absorbida en aire del LSCD

Energy Technology Data Exchange (ETDEWEB)

Alvarez R, M T; Tovar M, V M; Cejudo A, J [ININ, 52045 Ocoyoacac, Estado de Mexico (Mexico)

2005-12-15

determinations of the temperature to diminish their influence in the U. c. The percentage difference of the magnitudes dosemeters carried out by it patterns are consistent with U certain. However, it is necessary to diminish the uncertainty in the physical factors different to {kappa}{sub {tau}} and {sigma}{sub {beta}} for the one case of the primary patterns; because these they should be those of smaller value of U. d. In the case of the secondary patterns and tertiary for the realization of the{kappa}{sub {alpha}}{sub {center_dot}} is necessary to determine the corrections explicitly for recombination and polarization; and to analyze their contribution in the U. e. It is necessary to recover the tracking for the mensurations of the humidity. f. It is recommended to continue the control mensurations for each pattern, taking it{sup s} the least a measure every fifteen days, that it corresponds at two measured for month and 24 at the year. g. The operation of the air conditioned perturb the measurement for such as it recommends not to use it, and alone to leave in balance the chamber with the air of the engine room. (Author)

Determination of transference numbers in ionic conductors by the EMF method with active load

International Nuclear Information System (INIS)

Gorelov, V.P.

1988-01-01

Method for determining transference numbers in ionic conductors by means of measuring EMF of concentration cell with accout of polarization resistance of electrodes is suggested. The method enables to determine easily very small transference numbers of electron component against the background of predominating ionic conductivity. To illustrate the method there were determined transference numbers for the sample of industrial solid electrolyte in the cell; O 2 Pt|0.91ZrO 2 +0.09Y 2 O 3 |Pt, air

Unlocking the Full Potential of Extragalactic Lyα through Its Polarization Properties

Science.gov (United States)

Eide, Marius B.; Gronke, Max; Dijkstra, Mark; Hayes, Matthew

2018-04-01

Lyα is a powerful astrophysical probe. Not only is it ubiquitous at high redshifts, it is also a resonant line, making Lyα photons scatter. This scattering process depends on the physical conditions of the gas through which Lyα propagates, and these conditions are imprinted on observables such as the Lyα spectrum and its surface brightness profile. In this work, we focus on a less-used observable capable of probing any scattering process: polarization. We implement the density matrix formalism of polarization into the Monte Carlo radiative transfer code tlac. This allows us to treat it as a quantum mechanical process where single photons develop and lose polarization from scatterings in arbitrary gas geometries. We explore static and expanding ellipsoids, biconical outflows, and clumpy multiphase media. We find that photons become increasingly polarized as they scatter and diffuse into the wings of the line profiles, making scattered Lyα polarized in general. The degree and orientation of Lyα polarization depends on the kinematics and distribution of the scattering H I gas. We find that it generally probes spatial or velocity space asymmetries and aligns itself tangentially to the emission source. We show that the mentioned observables, when studied separately, can leave similar signatures for different source models. We conclude by revealing how a joint analysis of the Lyα spectra, surface brightness profiles, and polarization can break these degeneracies and help us extract unique physical information on galaxies and their environments from their strongest, most prominent emission line.

Evidence for the TICT mediated nonradiative deexcitation process for the excited coumarin-1 dye in high polarity protic solvents

Energy Technology Data Exchange (ETDEWEB)

Barik, Atanu [Radiation Chemistry and Chemical Dynamics Division, Bhabha Atomic Research Center, Trombay, Mumbai 400 085 (India); Kumbhakar, Manoj [Radiation Chemistry and Chemical Dynamics Division, Bhabha Atomic Research Center, Trombay, Mumbai 400 085 (India); Nath, Sukhendu [Radiation Chemistry and Chemical Dynamics Division, Bhabha Atomic Research Center, Trombay, Mumbai 400 085 (India); Pal, Haridas [Radiation Chemistry and Chemical Dynamics Division, Bhabha Atomic Research Center, Trombay, Mumbai 400 085 (India)

2005-08-29

Photophysical properties of coumarin-1 (C1) dye in different protic solvents have been investigated using steady-state and time-resolved fluorescence measurements. Correlation of the Stokes' shifts ({delta}{nu}-bar ) with the solvent polarity ({delta}f) suggests the intramolecular charge transfer (ICT) character for the dye fluorescent state. Fluorescence quantum yields ({phi}{sub f}) and lifetimes ({tau}{sub f}) of the dye show an abrupt reduction in high polarity solvents having {delta}f >{approx}0.28. In these solvents {tau}{sub f} is seen to be strongly temperature dependent, though it is temperature independent in solvents with {delta}f <{approx}0.28. It is inferred that in high polarity protic solvents there is a participation of an additional nonradiative decay process via the involvement of twisted intramolecular charge transfer (TICT) state. Unlike present results, no involvement of TICT state was observed even in strongly polar aprotic solvent like acetonitrile. It is indicated that the intermolecular hydrogen bonding of the dye with protic solvents in addition with the solvent polarity helps in the stabilization of the TICT state for C1 dye. Unlike most TICT molecules, the activation barrier ({delta}E{sub a}) for the TICT mediated nonradiative process for C1 dye is seen to increase with solvent polarity. This is rationalized on the basis of the assumption that the TICT to ground state conversion is the activation-controlled rate-determining step for the present system than the usual ICT to TICT conversion as encountered for most other TICT molecules.

Quantitative analysis of intramolecular exciplex and electron transfer in a double-linked zinc porphyrin-fullerene dyad.

Science.gov (United States)

Al-Subi, Ali Hanoon; Niemi, Marja; Tkachenko, Nikolai V; Lemmetyinen, Helge

2012-10-04

Photoinduced charge transfer in a double-linked zinc porphyrin-fullerene dyad is studied. When the dyad is excited at the absorption band of the charge-transfer complex (780 nm), an intramolecular exciplex is formed, followed by the complete charge separated (CCS) state. By analyzing the results obtained from time-resolved transient absorption and emission decay measurements in a range of solvents with different polarities, we derived a dependence between the observable lifetimes and internal parameters controlling the reaction rate constants based on the semiquantum Marcus electron-transfer theory. The critical value of the solvent polarity was found to be ε(r) ≈ 6.5: in solvents with higher dielectric constants, the energy of the CCS state is lower than that of the exciplex and the relaxation takes place via the CCS state predominantly, whereas in solvents with lower polarities the energy of the CCS state is higher and the exciplex relaxes directly to the ground state. In solvents with moderate polarities the exciplex and the CCS state are in equilibrium and cannot be separated spectroscopically. The degree of the charge shift in the exciplex relative to that in the CCS state was estimated to be 0.55 ± 0.02. The electronic coupling matrix elements for the charge recombination process and for the direct relaxation of the exciplex to the ground state were found to be 0.012 ± 0.001 and 0.245 ± 0.022 eV, respectively.

Polarization holography

DEFF Research Database (Denmark)

Nikolova, L.; Ramanujam, P.S.

Current research into holography is concerned with applications in optically storing, retrieving, and processing information. Polarization holography has many unique properties compared to conventional holography. It gives results in high efficiency, achromaticity, and special polarization...... properties. This books reviews the research carried out in this field over the last 15 years. The authors provide basic concepts in polarization and the propagation of light through anisotropic materials, before presenting a sound theoretical basis for polarization holography. The fabrication...... and characterization of azobenzene based materials, which remain the most efficient for the purpose, is described in detail. This is followed by a description of other materials that are used in polarization holography. An in-depth description of various applications, including display holography and optical storage...

Triplet superconductivity in PrOs{sub 4}Sb{sub 12}

Energy Technology Data Exchange (ETDEWEB)

Maki, K. [Department of Physics and Astronomy, University of Southern California, Los Angeles, CA 90089-0484 (United States); Won, H. [Department of Physics, Hallym University Chuncheon 200-702 (Korea, Republic of) ]. E-mail: hkwon@hallym.ac.kr; Parker, David [Department of Physics and Astronomy, University of Southern California, Los Angeles, CA 90089-0484 (United States); Haas, Stephan [Department of Physics and Astronomy, University of Southern California, Los Angeles, CA 90089-0484 (United States); Izawa, K. [Institute for Solid State Physics, University of Tokyo, Kashiwanoha, Kashiwa, Chiba 277-8581 (Japan); Matsuda, Y. [Institute for Solid State Physics, University of Tokyo, Kashiwanoha, Kashiwa, Chiba 277-8581 (Japan)

2005-04-30

Here we propose spin triplet superconductors for the A- and B-phase in PrOs{sub 4}Sb{sub 12}. The present model describes consistently the thermal conductivity {kappa}{sub zz} data obtained by Izawa et al. for T>=150mK.

Two-Dimensional Free Energy Surfaces for Electron Transfer Reactions in Solution

Directory of Open Access Journals (Sweden)

Shigeo Murata

2008-01-01

Full Text Available Change in intermolecular distance between electron donor (D and acceptor (A can induce intermolecular electron transfer (ET even in nonpolar solvent, where solvent orientational polarization is absent. This was shown by making simple calculations of the energies of the initial and final states of ET. In the case of polar solvent, the free energies are functions of both D-A distance and solvent orientational polarization. On the basis of 2-dimensional free energy surfaces, the relation of Marcus ET and exciplex formation is discussed. The transient effect in fluorescence quenching was measured for several D-A pairs in a nonpolar solvent. The results were analyzed by assuming a distance dependence of the ET rate that is consistent with the above model.

Polarized neutron spectrometer

International Nuclear Information System (INIS)

Abov, Yu.G.; Novitskij, V.V.; Alfimenkov, V.P.; Galinskij, E.M.; Mareev, Yu.D.; Pikel'ner, L.B.; Chernikov, A.N.; Lason', L.; Tsulaya, V.M.; Tsulaya, M.I.

2000-01-01

The polarized neutron spectrometer, intended for studying the interaction of polarized neutrons with nuclei and condensed media in the area of energies from thermal up to several electron-volt, is developed at the IBR-2 reactor (JINR, Dubna). Diffraction on the Co(92%)-Fe(8%) magnetized monocrystals is used for the neutron polarization and polarization analysis. The neutron polarization within the whole energy range equals ∼ 95% [ru

Modeling Polarized Emission from Black Hole Jets: Application to M87 Core Jet

Directory of Open Access Journals (Sweden)

Monika Mościbrodzka

2017-09-01

Full Text Available We combine three-dimensional general-relativistic numerical models of hot, magnetized Advection Dominated Accretion Flows around a supermassive black hole and the corresponding outflows from them with a general relativistic polarized radiative transfer model to produce synthetic radio images and spectra of jet outflows. We apply the model to the underluminous core of M87 galaxy. The assumptions and results of the calculations are discussed in context of millimeter observations of the M87 jet launching zone. Our ab initio polarized emission and rotation measure models allow us to address the constrains on the mass accretion rate onto the M87 supermassive black hole.

Control of Electronic Conduction at an Oxide Heterointerface using Surface Polar Adsorbates

Energy Technology Data Exchange (ETDEWEB)

Bell, Christopher

2011-08-19

We study the effect of the surface adsorption of a variety of common laboratory solvents on the conductivity at the interface between LaAlO{sub 3} and SrTiO{sub 3}. This interface possesses a range of intriguing physics, notably a proposed connection between the surface state of the LaAlO{sub 3} and the conductivity buried in the SrTiO{sub 3}. We show that the application of chemicals such as acetone, ethanol, and water can induce a large change (factor of three) in the conductivity. This phenomenon is observed only for polar solvents. These data provide experimental evidence for a general polarization-facilitated electronic transfer mechanism.

Study of charge transfer reactions in a microbial fuel cell

Energy Technology Data Exchange (ETDEWEB)

Martin, E.; Savadogo, O. [Ecole Polytechnique, Montreal, PQ (Canada). Dept. de Genie Chimique; National Research Council of Canada, Montreal, PQ (Canada). Biotechnology Research Inst.; Tartakovsky, B. [National Research Council of Canada, Montreal, PQ (Canada). Biotechnology Research Inst.

2008-07-01

Electron transfer reactions in a microbial fuel cell (MFC) were evaluated. The MFC was inoculated with anaerobic mesophilic sludge and operated with carbon felt, carbon cloth, and platinum (Pt) coated carbon cloth. The MFC was then fed with either acetate or glucose as a source of fuel and operated at a temperature of 25 degrees C and a pH of 7. Scanning electron microscopy (SEM) micrographs demonstrated that the micro-organisms colonized the anodes. Cyclic voltammetry and polarization tests were conducted using different fractions of the anodophilic biofilm in order to determine charge transfer routes. The study characterized the electron transfer mechanisms used by the exoelectrogenic micro-organisms to produce electricity. It was concluded that further research is needed to characterize reaction transfer routes. 2 refs., 1 fig.

PolarTrack: Optical Outside-In Device Tracking that Exploits Display Polarization

DEFF Research Database (Denmark)

Rädle, Roman; Jetter, Hans-Christian; Fischer, Jonathan

2018-01-01

PolarTrack is a novel camera-based approach to detecting and tracking mobile devices inside the capture volume. In PolarTrack, a polarization filter continuously rotates in front of an off-the-shelf color camera, which causes the displays of observed devices to periodically blink in the camera feed....... The periodic blinking results from the physical characteristics of current displays, which shine polarized light either through an LC overlay to produce images or through a polarizer to reduce light reflections on OLED displays. PolarTrack runs a simple detection algorithm on the camera feed to segment...... displays and track their locations and orientations, which makes PolarTrack particularly suitable as a tracking system for cross-device interaction with mobile devices. Our evaluation of PolarTrack's tracking quality and comparison with state-of-the-art camera-based multi-device tracking showed a better...

Electrochemical impedance spectroscopy investigation on indium tin oxide films under cathodic polarization in NaOH solution

International Nuclear Information System (INIS)

Gao, Wenjiao; Cao, Si; Yang, Yanze; Wang, Hao; Li, Jin; Jiang, Yiming

2012-01-01

The electrochemical corrosion behaviors of indium tin oxide (ITO) films under the cathodic polarization in 0.1 M NaOH solution were investigated by electrochemical impedance spectroscopy. The as-received and the cathodically polarized ITO films were characterized by scanning electron microscopy, energy dispersive X-ray spectroscopy and X-ray diffraction for morphological, compositional and structural studies. The results showed that ITO films underwent a corrosion process during the cathodic polarization and the main component of the corrosion products was body-centered cubic indium. The electrochemical impedance parameters were related to the effect of the cathodic polarization on the ITO specimens. The capacitance of ITO specimens increased, while the charge transfer resistance and the inductance decreased with the increase of the polarization time. The proposed mechanism indicated that the corrosion products (metallic indium) were firstly formed during the cathodic polarization and then absorbed on the surface of the ITO film. As the surface was gradually covered by indium particles, the corrosion process was suppressed. - Highlights: ► Cathodic polarization of indium tin oxide (ITO) in 0.1 M NaOH. ► Cathodic polarization studied with electrochemical impedance spectroscopy. ► ITO underwent a corrosion attack during cathodic polarization, indium was observed. ► Electrochemical parameters of ITO were obtained using equivalent electrical circuit. ► A corrosion mechanism is proposed.

Ligand and membrane-binding behavior of the phosphatidylinositol transfer proteins PITPα and PITPβ.

Science.gov (United States)

Baptist, Matilda; Panagabko, Candace; Cockcroft, Shamshad; Atkinson, Jeffrey

2016-12-01

Phosphatidylinositol transfer proteins (PITPs) are believed to be lipid transfer proteins because of their ability to transfer either phosphatidylinositol (PI) or phosphatidylcholine (PC) between membrane compartments, in vitro. However, the detailed mechanism of this transfer process is not fully established. To further understand the transfer mechanism of PITPs we examined the interaction of PITPs with membranes using dual polarization interferometry (DPI), which measures protein binding affinity on a flat immobilized lipid surface. In addition, a fluorescence resonance energy transfer (FRET)-based assay was also employed to monitor how quickly PITPs transfer their ligands to lipid vesicles. DPI analysis revealed that PITPβ had a higher affinity to membranes compared with PITPα. Furthermore, the FRET-based transfer assay revealed that PITPβ has a higher ligand transfer rate compared with PITPα. However, both PITPα and PITPβ demonstrated a preference for highly curved membrane surfaces during ligand transfer. In other words, ligand transfer rate was higher when the accepting vesicles were highly curved.

DVCS in the fragmentation region of polarized electron

International Nuclear Information System (INIS)

Akushevich, I.; Kuraev, E.A.; Nikolaev, N.N.

2000-01-01

For the kinematical region when a hard photon is emitted predominantly close to the direction of motion of a longitudinally polarized initial electron and relatively small momentum transfer to a proton we calculate the azimuthal asymmetry of a photon emission. It arises from the interference of the Bethe-Heitler amplitude and those which are described by a heavy photon impact factor. The azimuthal asymmetry does not decrease in the limit of infinite cms energy. The lowest order expression for the impact factor of a heavy photon is presented

Lunar true polar wander inferred from polar hydrogen.

Science.gov (United States)

Siegler, M A; Miller, R S; Keane, J T; Laneuville, M; Paige, D A; Matsuyama, I; Lawrence, D J; Crotts, A; Poston, M J

2016-03-24

The earliest dynamic and thermal history of the Moon is not well understood. The hydrogen content of deposits near the lunar poles may yield insight into this history, because these deposits (which are probably composed of water ice) survive only if they remain in permanent shadow. If the orientation of the Moon has changed, then the locations of the shadowed regions will also have changed. The polar hydrogen deposits have been mapped by orbiting neutron spectrometers, and their observed spatial distribution does not match the expected distribution of water ice inferred from present-day lunar temperatures. This finding is in contrast to the distribution of volatiles observed in similar thermal environments at Mercury's poles. Here we show that polar hydrogen preserves evidence that the spin axis of the Moon has shifted: the hydrogen deposits are antipodal and displaced equally from each pole along opposite longitudes. From the direction and magnitude of the inferred reorientation, and from analysis of the moments of inertia of the Moon, we hypothesize that this change in the spin axis, known as true polar wander, was caused by a low-density thermal anomaly beneath the Procellarum region. Radiogenic heating within this region resulted in the bulk of lunar mare volcanism and altered the density structure of the Moon, changing its moments of inertia. This resulted in true polar wander consistent with the observed remnant polar hydrogen. This thermal anomaly still exists and, in part, controls the current orientation of the Moon. The Procellarum region was most geologically active early in lunar history, which implies that polar wander initiated billions of years ago and that a large portion of the measured polar hydrogen is ancient, recording early delivery of water to the inner Solar System. Our hypothesis provides an explanation for the antipodal distribution of lunar polar hydrogen, and connects polar volatiles to the geologic and geophysical evolution of the Moon

Super-Planckian far-field radiative heat transfer

Science.gov (United States)

Fernández-Hurtado, V.; Fernández-Domínguez, A. I.; Feist, J.; García-Vidal, F. J.; Cuevas, J. C.

2018-01-01

We present here a theoretical analysis that demonstrates that the far-field radiative heat transfer between objects with dimensions smaller than the thermal wavelength can overcome the Planckian limit by orders of magnitude. To guide the search for super-Planckian far-field radiative heat transfer, we make use of the theory of fluctuational electrodynamics and derive a relation between the far-field radiative heat transfer and the directional absorption efficiency of the objects involved. Guided by this relation, and making use of state-of-the-art numerical simulations, we show that the far-field radiative heat transfer between highly anisotropic objects can largely overcome the black-body limit when some of their dimensions are smaller than the thermal wavelength. In particular, we illustrate this phenomenon in the case of suspended pads made of polar dielectrics like SiN or SiO2. These structures are widely used to measure the thermal transport through nanowires and low-dimensional systems and can be employed to test our predictions. Our work illustrates the dramatic failure of the classical theory to predict the far-field radiative heat transfer between micro- and nanodevices.

Polarized proton beams

International Nuclear Information System (INIS)

Roser, T.

1995-01-01

The acceleration of polarized proton beams in circular accelerators is complicated by the presence of numerous depolarizing spin resonances. Careful and tedious minimization of polarization loss at each of these resonances allowed acceleration of polarized proton beams up to 22 GeV. It has been the hope that Siberian Snakes, which are local spin rotators inserted into ring accelerators, would eliminate these resonances and allow acceleration of polarized beams with the same ease and efficiency that is now routine for unpolarized beams. First tests at IUCF with a full Siberian Snake showed that the spin dynamics with a Snake can be understood in detail. The author now has results of the first tests of a partial Siberian Snake at the AGS, accelerating polarized protons to an energy of about 25 GeV. These successful tests of storage and acceleration of polarized proton beams open up new possibilities such as stored polarized beams for internal target experiments and high energy polarized proton colliders

Climate impact of idealized winter polar mesospheric and stratospheric ozone losses as caused by energetic particle precipitation

Science.gov (United States)

Meraner, Katharina; Schmidt, Hauke

2018-01-01

Energetic particles enter the polar atmosphere and enhance the production of nitrogen oxides and hydrogen oxides in the winter stratosphere and mesosphere. Both components are powerful ozone destroyers. Recently, it has been inferred from observations that the direct effect of energetic particle precipitation (EPP) causes significant long-term mesospheric ozone variability. Satellites observe a decrease in mesospheric ozone up to 34 % between EPP maximum and EPP minimum. Stratospheric ozone decreases due to the indirect effect of EPP by about 10-15 % observed by satellite instruments. Here, we analyze the climate impact of winter boreal idealized polar mesospheric and polar stratospheric ozone losses as caused by EPP in the coupled Max Planck Institute Earth System Model (MPI-ESM). Using radiative transfer modeling, we find that the radiative forcing of mesospheric ozone loss during polar night is small. Hence, climate effects of mesospheric ozone loss due to energetic particles seem unlikely. Stratospheric ozone loss due to energetic particles warms the winter polar stratosphere and subsequently weakens the polar vortex. However, those changes are small, and few statistically significant changes in surface climate are found.

GAUSS-SEIDEL AND SUCCESSIVE OVERRELAXATION METHODS FOR RADIATIVE TRANSFER WITH PARTIAL FREQUENCY REDISTRIBUTION

International Nuclear Information System (INIS)

Sampoorna, M.; Bueno, J. Trujillo

2010-01-01

The linearly polarized solar limb spectrum that is produced by scattering processes contains a wealth of information on the physical conditions and magnetic fields of the solar outer atmosphere, but the modeling of many of its strongest spectral lines requires solving an involved non-local thermodynamic equilibrium radiative transfer problem accounting for partial redistribution (PRD) effects. Fast radiative transfer methods for the numerical solution of PRD problems are also needed for a proper treatment of hydrogen lines when aiming at realistic time-dependent magnetohydrodynamic simulations of the solar chromosphere. Here we show how the two-level atom PRD problem with and without polarization can be solved accurately and efficiently via the application of highly convergent iterative schemes based on the Gauss-Seidel and successive overrelaxation (SOR) radiative transfer methods that had been previously developed for the complete redistribution case. Of particular interest is the Symmetric SOR method, which allows us to reach the fully converged solution with an order of magnitude of improvement in the total computational time with respect to the Jacobi-based local accelerated lambda iteration method.

Gauss-Seidel and Successive Overrelaxation Methods for Radiative Transfer with Partial Frequency Redistribution

Science.gov (United States)

Sampoorna, M.; Trujillo Bueno, J.

2010-04-01

The linearly polarized solar limb spectrum that is produced by scattering processes contains a wealth of information on the physical conditions and magnetic fields of the solar outer atmosphere, but the modeling of many of its strongest spectral lines requires solving an involved non-local thermodynamic equilibrium radiative transfer problem accounting for partial redistribution (PRD) effects. Fast radiative transfer methods for the numerical solution of PRD problems are also needed for a proper treatment of hydrogen lines when aiming at realistic time-dependent magnetohydrodynamic simulations of the solar chromosphere. Here we show how the two-level atom PRD problem with and without polarization can be solved accurately and efficiently via the application of highly convergent iterative schemes based on the Gauss-Seidel and successive overrelaxation (SOR) radiative transfer methods that had been previously developed for the complete redistribution case. Of particular interest is the Symmetric SOR method, which allows us to reach the fully converged solution with an order of magnitude of improvement in the total computational time with respect to the Jacobi-based local accelerated lambda iteration method.

Wireless Power Transfer to a Microaerial Vehicle with a Microwave Active Phased Array

Directory of Open Access Journals (Sweden)

Shotaro Nako

2014-01-01

Full Text Available A wireless power transfer system using a microwave active phased array was developed. In the system, power is transferred to a circling microaerial vehicle (MAV by a microwave beam of 5.8 GHz, which is formed and directed to the MAV using an active phased array antenna. The MAV is expected to support observation of areas that humans cannot reach. The power beam is formed by the phased array with eight antenna elements. Input power is about 5.6 W. The peak power density at 1,500 mm altitude was 2.63 mW/cm2. The power is sent to a circling MAV. Therefore, the transfer beam should be polarized circularly to achieve a constant power supply independent of its yaw angle. To minimize the polarization loss, a sequentially routed antenna (SRA was applied to the transmitter antenna. Results show that the axial ratio of 0.440 dB was accomplished and that power fluctuation was kept below 1%.

Titanium magnetic polarization at the Fe/BaTiO3 interfaces: An effect of ferroelectric polarization discontinuity

Science.gov (United States)

Paul, Amitesh; Zheng, Jian-Guo; Aoki, Toshihiro

2017-10-01

The exotic magnetic phenomena and the associated functionalities have attracted extensive scientific interest in fundamental physics and cater to the purpose of the novel material search. In this article, with a combination of the electron energy-loss spectroscopy and the X-ray absorption spectroscopy, we have investigated the interfacial Fe atoms and the induced ferromagnetic moment of Ti atoms in Fe/BaTiO3 (BTO) heterostructures. The samples were grown with two different BTO thicknesses, thus resulting in two different states of distorted oxygen environments or different electrostatic potentials. We demonstrate that in these systems, the electronic and magnetic proximity effects remain coupled as the ferroelectric polar discontinuity is held responsible for an induced transfer of the interface electrons. These electrons migrate from the Fe2+ layers to the Ti(4+)-δ layers with the hybridization via O-2p oxide orbitals into Ti orbitals to screen the ferroelectric polarization. These findings, in charge neutral BaO-TiO2 and FeO layers or nonpolar/nopolar interface, essentially underline the central role of the covalent bonding in defining the spin-electronic properties.

A Novel Approach to Exploring the Mars Polar Caps

Science.gov (United States)

Brophy, John R.; Carsey, Frank D.; Rodgers, David H.; Soderblom, L. A.; Wilcox, Brian H.

2000-01-01

The Martian polar caps contain some of the most important scientific sites on the planet. There is much interest in exploring them with a view to understanding their role in the Mars climate system. By gaining access to the stratigraphy of the polar terrain, it is probable that one can access the climate history of the planet. Additionally, investigations aimed at localizing subsurface water--liquid or solid--are not only of great scientific interest but are also germane to the long-term interests of the manned space flight program. A major difficulty with polar exploration is access. Current techniques using chemical propulsion, Holman transfers, and direct-entry landers with aeroshells have limited capability to access the polar terrain. For the near term the authors propose a new approach to solving this transportation issue by using Solar Electric Propulsion (SEP), recently flight demonstrated on NASA's DS1 Mission to an asteroid and a comet. For a longer-term approach there are additional ways in which access to Mars, as well as other planets, can be significantly improved. These include the use of Chaos orbit theory to enable transportation between LaGrange points in the solar system, gossamer structures enabling very low-mass mobility, and advanced ascent vehicles. In this paper the authors describe how a 1000-kG payload can be transported to the surface of Mars and a polar sample obtained and returned to Earth in less than five years using SEP. A vision of how this approach can be integrated into a long-term Mars exploration strategy building toward the future is also discussed.

A Novel Approach to Exploring the Mars Polar Caps

Science.gov (United States)

Brophy, John R.; Carsey, Frank D.; Rodgers, David H.; Soderblom, L. A.; Wilcox, Brian H.

2000-08-01

The Martian polar caps contain some of the most important scientific sites on the planet. There is much interest in exploring them with a view to understanding their role in the Mars climate system. By gaining access to the stratigraphy of the polar terrain, it is probable that one can access the climate history of the planet. Additionally, investigations aimed at localizing subsurface water--liquid or solid--are not only of great scientific interest but are also germane to the long-term interests of the manned space flight program. A major difficulty with polar exploration is access. Current techniques using chemical propulsion, Holman transfers, and direct-entry landers with aeroshells have limited capability to access the polar terrain. For the near term the authors propose a new approach to solving this transportation issue by using Solar Electric Propulsion (SEP), recently flight demonstrated on NASA's DS1 Mission to an asteroid and a comet. For a longer-term approach there are additional ways in which access to Mars, as well as other planets, can be significantly improved. These include the use of Chaos orbit theory to enable transportation between LaGrange points in the solar system, gossamer structures enabling very low-mass mobility, and advanced ascent vehicles. In this paper the authors describe how a 1000-kG payload can be transported to the surface of Mars and a polar sample obtained and returned to Earth in less than five years using SEP. A vision of how this approach can be integrated into a long-term Mars exploration strategy building toward the future is also discussed.

Transfer and conversion of images based on EIT in atom vapor.

Science.gov (United States)

Cao, Mingtao; Zhang, Liyun; Yu, Ya; Ye, Fengjuan; Wei, Dong; Guo, Wenge; Zhang, Shougang; Gao, Hong; Li, Fuli

2014-05-01

Transfer and conversion of images between different wavelengths or polarization has significant applications in optical communication and quantum information processing. We demonstrated the transfer of images based on electromagnetically induced transparency (EIT) in a rubidium vapor cell. In experiments, a 2D image generated by a spatial light modulator is used as a coupling field, and a plane wave served as a signal field. We found that the image carried by coupling field could be transferred to that carried by signal field, and the spatial patterns of transferred image are much better than that of the initial image. It also could be much smaller than that determined by the diffraction limit of the optical system. We also studied the subdiffraction propagation for the transferred image. Our results may have applications in quantum interference lithography and coherent Raman spectroscopy.

Charge transport in non-polar and semi-polar III-V nitride heterostructures

International Nuclear Information System (INIS)

Konar, Aniruddha; Verma, Amit; Fang, Tian; Zhao, Pei; Jana, Raj; Jena, Debdeep

2012-01-01

Compared to the intense research focus on the optical properties, the transport properties in non-polar and semi-polar III-nitride semiconductors remain relatively unexplored to date. The purpose of this paper is to discuss charge-transport properties in non-polar and semi-polar orientations of GaN in a comparative fashion to what is known for transport in polar orientations. A comprehensive approach is adopted, starting from an investigation of the differences in the electronic bandstructure along different polar orientations of GaN. The polarization fields along various orientations are then discussed, followed by the low-field electron and hole mobilities. A number of scattering mechanisms that are specific to non-polar and semi-polar GaN heterostructures are identified, and their effects are evaluated. Many of these scattering mechanisms originate due to the coupling of polarization with disorder and defects in various incarnations depending on the crystal orientation. The effect of polarization orientation on carrier injection into quantum-well light-emitting diodes is discussed. This paper ends with a discussion of orientation-dependent high-field charge-transport properties including velocity saturation, instabilities and tunneling transport. Possible open problems and opportunities are also discussed. (paper)

Hydrogen-transfer and charge-transfer in photochemical and radiation induced reactions. Progress report, November 1, 1975--October 31, 1976

International Nuclear Information System (INIS)

Cohen, S.G.

1976-10-01

The relative importance of light absorption, quenching of triplet, and hydrogen transfer repair has been examined in retardation by mercaptans of photoreduction of aromatic ketones by alcohols. In the reduction of benzophenone by 2-propanol, retardation is efficient and, after correction for the first two effects, is due entirely to hydrogen-transfer repair, as indicated by deuterium labeling. In reduction of acetophenone by α-methylbenzyl alcohol, repair by hydrogen transfer is also operative. In reduction of benzophenone by benzhydrol, retardation is less efficient and is due to quenching, as the ketyl radical does not abstract hydrogen from mercaptan rapidly in competition with coupling. Deuterium isotope effects are discussed in terms of competitive reactions. Photoreduction of benzophenone by 2-butylamine and by triethylamine is retarded by aromatic mercaptans and disulfides. Of the retardation not due to light absorption and triplet quenching by the sulfur compounds, half is due to hydrogen-transfer repair, as indicated by racemization and deuterium labeling. The remainder is attributed to quenching by the sulfur compound of the charge-transfer-complex intermediate. Photoreduction by primary and secondary amines, but not by tertiary amines, is accelerated by aliphatic mercaptans. The acceleration is attributed to catalysis of hydrogen transfer by the mercaptan in the charge-transfer complex. The effect is large in hydrocarbon solvent, less in polar organic solvents and absent in water

Polarization-sensitive color in butterfly scales: polarization conversion from ridges with reflecting elements.

Science.gov (United States)

Zhang, Ke; Tang, Yiwen; Meng, Jinsong; Wang, Ge; Zhou, Han; Fan, Tongxiang; Zhang, Di

2014-11-03

Polarization-sensitive color originates from polarization-dependent reflection or transmission, exhibiting abundant light information, including intensity, spectral distribution, and polarization. A wide range of butterflies are physiologically sensitive to polarized light, but the origins of polarized signal have not been fully understood. Here we systematically investigate the colorful scales of six species of butterfly to reveal the physical origins of polarization-sensitive color. Microscopic optical images under crossed polarizers exhibit their polarization-sensitive characteristic, and micro-structural characterizations clarify their structural commonality. In the case of the structural scales that have deep ridges, the polarization-sensitive color related with scale azimuth is remarkable. Periodic ridges lead to the anisotropic effective refractive indices in the parallel and perpendicular grating orientations, which achieves form-birefringence, resulting in the phase difference of two different component polarized lights. Simulated results show that ridge structures with reflecting elements reflect and rotate the incident p-polarized light into s-polarized light. The dimensional parameters and shapes of grating greatly affect the polarization conversion process, and the triangular deep grating extends the outstanding polarization conversion effect from the sub-wavelength period to the period comparable to visible light wavelength. The parameters of ridge structures in butterfly scales have been optimized to fulfill the polarization-dependent reflection for secret communication. The structural and physical origin of polarization conversion provides a more comprehensive perspective on the creation of polarization-sensitive color in butterfly wing scales. These findings show great potential in anti-counterfeiting technology and advanced optical material design.

Ratiometric fluorescence polarization as a cytometric functional parameter: theory and practice

International Nuclear Information System (INIS)

Yishai, Yitzhak; Fixler, Dror; Cohen-Kashi, Meir; Zurgil, Naomi; Deutsch, Mordechai

2003-01-01

The use of ratiometric fluorescence polarization (RFP) as a functional parameter in monitoring cellular activation is suggested, based on the physical phenomenon of fluorescence polarization dependency on emission wavelengths in multiple (at least binary) solutions. The theoretical basis of this dependency is thoroughly discussed and examined via simulation. For simulation, aimed to imitate a fluorophore-stained cell, real values of the fluorescence spectrum and polarization of different single fluorophore solutions were used. The simulation as well as the experimentally obtained values of RFP indicated the high sensitivity of this measure. Finally, the RFP parameter was utilized as a cytometric measure in three exemplary cellular bioassays. In the first, the apoptotic effect of oxLDL in a human Jurkat FDA-stained T cell line was monitored by RFP. In the second, the interaction between cell surface membrane receptors of human T lymphocyte cells was monitored by RFP measurements as a complementary means to the fluorescence resonance energy transfer (FRET) technique. In the third bioassay, cellular thiol level of FDA- and CMFDA-labelled Jurkat T cells was monitored via RFP

System for measuring the proton polarization in a polarized target

International Nuclear Information System (INIS)

Karnaukhov, I.M.; Lukhanin, A.A.; Telegin, Yu.N.; Trotsenko, V.I.; Chechetenko, V.F.

1984-01-01

The system for measuring the proton polarization in a polarized target representing the high-sensitivity nuclear magnetic resonance (NMR) is described Q-meter with series connection and a circuit for measuring system resonance characteristic is used for NMR-absorption signal recording. Measuring coil is produced of a strip conductor in order to obtain uniform system sensitivity to polarization state in all target volume and improve signal-to-noise ratio. Polarization measuring system operates ion-line with the M-6000 computer. The total measuring error for the value of free proton polarization in target taking into account the error caused by local depolarization of working substance under irradiation by high-intense photon beam is <= 6%. Long-term application of the described system for measuring the proton polarization in the LUEh-20000 accelerator target used in the pion photoproduction experiments has demonstrated its high reliability

Sources of polarized neutrons

International Nuclear Information System (INIS)

Walter, L.

1983-01-01

Various sources of polarized neutrons are reviewed. Monoenergetic source produced with unpolarized or polarized beams, white sources of polarized neutrons, production by transmissions through polarized hydrogen targets and polarized thermal neutronsare discussed, with appropriate applications included. (U.K.)

Vacuum polarization in Coulomb field revisited

Energy Technology Data Exchange (ETDEWEB)

Zamastil, J., E-mail: zamastil@karlov.mff.cuni.cz; Šimsa, D.

2017-04-15

Simplified derivation of Wichmann–Kroll term is presented. The derivation uses two formulas for hypergeometric functions, but otherwise is elementary. It is found that Laplace transform of the vacuum charge density diverges at zero momentum transfer. This divergence has nothing to do with known ultraviolet divergence. The latter is related to the large momentum behavior of the pertinent integral, while the former to the small momentum behavior. When these divergences are removed, the energy shift caused by vacuum polarization for an ordinary hydrogen obtained here is in an exact agreement with the result obtained by Wichmann and Kroll. Also, for muonic hydrogen the result obtained here reasonably agrees with that given in literature.

Polarization observables measured in the reaction vector pp → pK{sup +}Λ by COSY-TOF

Energy Technology Data Exchange (ETDEWEB)

Hauenstein, Florian [Forschungszentrum Juelich, Juelich (Germany); Collaboration: COSY-TOF-Collaboration

2016-07-01

The vector pp → pK{sup +}Λ reaction was measured with the COSY-TOF detector using a polarized proton beam with beam momenta 2.7 GeV/c and 2.95 GeV/c. The measurements with a polarized beam allow the determination of polarization observables in addition to the differential cross sections. These observables are the Λ polarization, the spin transfer to the Λ and the analyzing power of the final state particles. The latter is connected with the partial wave composition of the final state system, while the first two can improve the understanding of the underlying reaction mechanism of the associated strangeness production. Currently, no sophisticated models exist in this energy regime, thus, conclusive results concerning the reaction mechanism can not be drawn yet. Nevertheless, the obtained data are the first with full phase space acceptance and high statistics in this beam energy regime. In this talk the extraction methods for the different polarization observables are explained, and results for the polarization observables as a function of different variables are shown. The dependencies of the results on the beam momentum are discussed. Furthermore, a comparison with theoretical expectations from high energy physics for the Λ polarization is given.

PolarHub: A Global Hub for Polar Data Discovery

Science.gov (United States)

Li, W.

2014-12-01

This paper reports the outcome of a NSF project in developing a large-scale web crawler PolarHub to discover automatically the distributed polar dataset in the format of OGC web services (OWS) in the cyberspace. PolarHub is a machine robot; its goal is to visit as many webpages as possible to find those containing information about polar OWS, extract this information and store it into the backend data repository. This is a very challenging task given huge data volume of webpages on the Web. Three unique features was introduced in PolarHub to make it distinctive from earlier crawler solutions: (1) a multi-task, multi-user, multi-thread support to the crawling tasks; (2) an extensive use of thread pool and Data Access Object (DAO) design patterns to separate persistent data storage and business logic to achieve high extendibility of the crawler tool; (3) a pattern-matching based customizable crawling algorithm to support discovery of multi-type geospatial web services; and (4) a universal and portable client-server communication mechanism combining a server-push and client pull strategies for enhanced asynchronous processing. A series of experiments were conducted to identify the impact of crawling parameters to the overall system performance. The geographical distribution pattern of all PolarHub identified services is also demonstrated. We expect this work to make a major contribution to the field of geospatial information retrieval and geospatial interoperability, to bridge the gap between data provider and data consumer, and to accelerate polar science by enhancing the accessibility and reusability of adequate polar data.

Polarization extinction ratio of the polarization crosstalk caused by point pressure force in the polarization-maintaining fiber

Science.gov (United States)

Mukhtubayev, Azamat B.; Aksarin, Stanislav M.; Strigalev, Vladimir E.

2017-11-01

A study of the orthogonal polarization modes crosstalk changes in the point of different mechanical actions (pressure force) in the polarization-maintaining fiber with straining elliptical cladding is presented. It was found that by increasing of the pressure force the polarization extinction ratio increases nonlinearly. Also revealed the dependence of the extinction coefficient and the angle between vector of the mechanical action and polarization axes of the test fiber, which leads to change the extinction coefficient variable from -57 dB to -25 dB under the pressure force of 0.7 N. Also it was found that the cross angle of the fiber axes doesn't influence on the extinction ratio value of the mechanical induced polarization crosstalk.

Polarized secondary radioactive beams

International Nuclear Information System (INIS)

Zaika, N.I.

1992-01-01

Three methods of polarized radioactive nuclei beam production: a) a method nuclear interaction of the non-polarized or polarized charged projectiles with target nuclei; b) a method of polarization of stopped reaction radioactive products in a special polarized ion source with than following acceleration; c) a polarization of radioactive nuclei circulating in a storage ring are considered. Possible life times of the radioactive ions for these methods are determined. General schemes of the polarization method realizations and depolarization problems are discussed

Photodissociation and charge transfer dynamics of negative ions studied with femtosecond photoelectron spectroscopy

Energy Technology Data Exchange (ETDEWEB)

Zanni, Martin Thomas [Univ. of California, Berkeley, CA (United States)

1999-12-01

This dissertation presents studies aimed at understanding the potential energy surfaces and dynamics of isolated negative ions, and the effects of solvent on each. Although negative ions play important roles in atmospheric and solution phase chemistry, to a large extent the ground and excited state potential energy surfaces of gas phase negative ions are poorly characterized, and solvent effects even less well understood. In an effort to fill this gap, the author's coworkers and the author have developed a new technique, anion femtosecond photoelectron spectroscopy, and applied it to gas phase photodissociation and charge transfer processes. Studies are presented that (1) characterize the ground and excited states of isolated and clustered anions, (2) monitor the photodissociation dynamics of isolated and clustered anions, and (3) explore the charge-transfer-to-solvent states of atomic iodide clustered with polar and non-polar solvents.

Photodissociation and charge transfer dynamics of negative ions studied with femtosecond photoelectron spectroscopy

International Nuclear Information System (INIS)

Zanni, Martin T.

1999-01-01

This dissertation presents studies aimed at understanding the potential energy surfaces and dynamics of isolated negative ions, and the effects of solvent on each. Although negative ions play important roles in atmospheric and solution phase chemistry, to a large extent the ground and excited state potential energy surfaces of gas phase negative ions are poorly characterized, and solvent effects even less well understood. In an effort to fill this gap, the author's coworkers and the author have developed a new technique, anion femtosecond photoelectron spectroscopy, and applied it to gas phase photodissociation and charge transfer processes. Studies are presented that (1) characterize the ground and excited states of isolated and clustered anions, (2) monitor the photodissociation dynamics of isolated and clustered anions, and (3) explore the charge-transfer-to-solvent states of atomic iodide clustered with polar and non-polar solvents

Visualization of Excitonic Structure in the Fenna-Matthews-Olson Photosynthetic Complex by Polarization-Dependent Two-Dimensional Electronic Spectroscopy

International Nuclear Information System (INIS)

Fleming, Graham; Read, Elizabeth L.; Schlau-Cohen, Gabriela S.; Engel, Gregory S.; Wen, Jianzhong; Blankenship, Robert E.; Fleming, Graham R.

2008-01-01

Photosynthetic light-harvesting proceeds by the collection and highly efficient transfer of energy through a network of pigment-protein complexes. Inter-chromophore electronic couplings and interactions between pigments and the surrounding protein determine energy levels of excitonic states and dictate the mechanism of energy flow. The excitonic structure (orientation of excitonic transition dipoles) of pigment-protein complexes is generally deduced indirectly from x-ray crystallography in combination with predictions of transition energies and couplings in the chromophore site basis. Here, we demonstrate that coarse-grained excitonic structural information in the form of projection angles between transition dipole moments can be obtained from polarization-dependent two-dimensional electronic spectroscopy of an isotropic sample, particularly when the nonrephasing or free polarization decay signal rather than the photon echo signal is considered. The method provides an experimental link between atomic and electronic structure and accesses dynamical information with femtosecond time resolution. In an investigation of the Fenna-Matthews-Olson complex from green sulfur bacteria, energy transfer connecting two particular exciton states in the protein is isolated as being the primary contributor to a cross peak in the nonrephasing 2D spectrum at 400 fs under a specific sequence of polarized excitation pulses. The results suggest the possibility of designing experiments using combinations of tailored polarization sequences to separate and monitor individual relaxation pathways

Scattering of polarized electrons from polarized targets: Coincidence reactions and prescriptions for polarized half-off-shell single-nucleon cross sections

International Nuclear Information System (INIS)

Caballero, J.A.; Massachusetts Inst. of Tech., Cambridge, MA; Donnelly, T.W.; Massachusetts Inst. of Tech., Cambridge, MA; Poulis, G.I.; Massachusetts Inst. of Tech., Cambridge, MA

1993-01-01

Coincidence reactions of the type vector A( vector e, e'N)B involving the scattering of polarized electrons from polarized targets are discussed within the context of the plane-wave impulse approximation. Prescriptions are developed for polarized half-off single-nucleon cross sections; the different prescriptions are compared for typical quasi-free kinematics. Illustrative results are presented for coincidence polarized electron scattering from typical polarized nuclei. (orig.)

Strategies to enhance the excitation energy-transfer efficiency in a light-harvesting system using the intra-molecular charge transfer character of carotenoids

Energy Technology Data Exchange (ETDEWEB)

Yukihira, Nao [Department of Applied Chemistry for Environment; School of Science and Technology; Kwansei Gakuin University; Sanda; Japan; Sugai, Yuko [Department of Applied Chemistry for Environment; School of Science and Technology; Kwansei Gakuin University; Sanda; Japan; Fujiwara, Masazumi [Department of Applied Chemistry for Environment; School of Science and Technology; Kwansei Gakuin University; Sanda; Japan; Kosumi, Daisuke [Institute of Pulsed Power Science; Kumamoto University; Kumamoto; Japan; Iha, Masahiko [South Product Co. Ltd.; Uruma-shi; Japan; Sakaguchi, Kazuhiko [Department of Chemistry; Graduate School of Science; Osaka City University; Osaka 558-8585; Japan; Katsumura, Shigeo [Department of Chemistry; Graduate School of Science; Osaka City University; Osaka 558-8585; Japan; Gardiner, Alastair T. [Glasgow Biomedical Research Centre; University of Glasgow; 126 University Place; Glasgow, G12 8QQ; UK; Cogdell, Richard J. [Glasgow Biomedical Research Centre; University of Glasgow; 126 University Place; Glasgow, G12 8QQ; UK; Hashimoto, Hideki [Department of Applied Chemistry for Environment; School of Science and Technology; Kwansei Gakuin University; Sanda; Japan

2017-01-01

Fucoxanthin is a carotenoid that is mainly found in light-harvesting complexes from brown algae and diatoms. Due to the presence of a carbonyl group attached to polyene chains in polar environments, excitation produces an excited intra-molecular charge transfer. This intra-molecular charge transfer state plays a key role in the highly efficient (~95%) energy-transfer from fucoxanthin to chlorophyllain the light-harvesting complexes from brown algae. In purple bacterial light-harvesting systems the efficiency of excitation energy-transfer from carotenoids to bacteriochlorophylls depends on the extent of conjugation of the carotenoids. In this study we were successful, for the first time, in incorporating fucoxanthin into a light-harvesting complex 1 from the purple photosynthetic bacterium,Rhodospirillum rubrumG9+ (a carotenoidless strain). Femtosecond pump-probe spectroscopy was applied to this reconstituted light-harvesting complex in order to determine the efficiency of excitation energy-transfer from fucoxanthin to bacteriochlorophyllawhen they are bound to the light-harvesting 1 apo-proteins.

Polarization dependence of the spin-density-wave excitations in single-domain chromium

Energy Technology Data Exchange (ETDEWEB)

Boeni, P. [Paul Scherrer Inst. (PSI), Villigen (Switzerland); Roessli, B. [Institut Max von Laue - Paul Langevin, 75 - Paris (France); Sternlieb, B.J. [Brookhaven (United States); Lorenzo, E. [Centre National de la Recherche Scientifique (CNRS), 38 - Grenoble (France); Werner, S.A. [Missouri (United States)

1997-09-01

A polarized neutron scattering experiment has been performed with a single-Q, single domain sample of chromium in a magnetic field of 4 T. It is confirmed that the longitudinal fluctuations are enhanced for small energy transfers and that the spin wave modes with {delta}S parallel to Q and {delta}S perpendicular to Q are similar. (author) 2 figs., 1 tab., 2 refs.

Measurement of the proton form factor ratio at low momentum transfer

Energy Technology Data Exchange (ETDEWEB)

Friedman, Moshe [Hebrew Univ. of Jerusalem (Israel)

2016-08-01

Experiment E08-007-II measured the proton elastic form factor ratio μG_E=G_M in the momentum transfer range of Q² ~ 0.02 - 0.08 GeV², the lowest ever measured by polarization transfer techniques. The experiment was performed at the Thomas Jefferson National Accelerator Facility in Newport News, Virginia, USA during 2012. A polarized electron beam with energies of 1.1, 1.7, and 2.2 GeV was elastically scattered off a polarized solid NH₃ target. The asymmetries between the cross section of positive and negative helicity states of the beam were determined. These asymmetries can be used to determine the form factor ratio. In this thesis, we present the asymmetry analysis of the experiment, discuss the main challenges and show preliminary results for part of the data. Preliminary asymmetries indicate an increase in the form factor ratio above unity. However, a complete analysis is required before any conclusion can be made. Further analysis is ongoing, and final asymmetry results and form factor extraction is expected during 2017. We also present first results for ¹⁴N asymmetries for elastic and quasi-elastic scattering. The measured asymmetries are in agreement with the shell model approximation, within the low accuracy of the measurement. A change in the asymmetry sign between the elastic and the quasi-elastic processes is seen, and should motivate further theoretical studies. These experimental asymmetries will also be useful for systematic studies of other experiments using polarized NH₃ targets.

Ortho-Babinet polarization-interrogating filter: an interferometric approach to polarization measurement.

Science.gov (United States)

Van Delden, Jay S

2003-07-15

A novel, interferometric, polarization-interrogating filter assembly and method for the simultaneous measurement of all four Stokes parameters across a partially polarized irradiance image in a no-moving-parts, instantaneous, highly sensitive manner is described. In the reported embodiment of the filter, two spatially varying linear retarders and a linear polarizer comprise an ortho-Babinet, polarization-interrogating (OBPI) filter. The OBPI filter uniquely encodes the incident ensemble of electromagnetic wave fronts comprising a partially polarized irradiance image in a controlled, deterministic, spatially varying manner to map the complete state of polarization across the image to local variations in a superposed interference pattern. Experimental interferograms are reported along with a numerical simulation of the method.

Coronal Polarization of Pseudostreamers and the Solar Polar Field Reversal

Science.gov (United States)

Rachmeler, L. A.; Guennou, C.; Seaton, D. B.; Gibson, S. E.; Auchere, F.

2016-01-01

The reversal of the solar polar magnetic field is notoriously hard to pin down due to the extreme viewing angle of the pole. In Cycle 24, the southern polar field reversal can be pinpointed with high accuracy due to a large-scale pseudostreamer that formed over the pole and persisted for approximately a year. We tracked the size and shape of this structure with multiple observations and analysis techniques including PROBA2/SWAP EUV images, AIA EUV images, CoMP polarization data, and 3D tomographic reconstructions. We find that the heliospheric field reversed polarity in February 2014, whereas in the photosphere, the last vestiges of the previous polar field polarity remained until March 2015. We present here the evolution of the structure and describe its identification in the Fe XII 1074nm coronal emission line, sensitive to the Hanle effect in the corona.

Experiments with Fermilab polarized proton and polarized antiproton beams

International Nuclear Information System (INIS)

Yokosawa, A.

1990-01-01

We summarize activities concerning the Fermilab polarized beams. They include a brief description of the polarized-beam facility, measurements of beam polarization by polarimeters, asymmetry measurements in the π degree production at high p perpendicular and in the Λ (Σ degree), π ± , π degree production at large x F , and Δσ L (pp, bar pp) measurements. 18 refs

Measurements of the spin structure of the nucleon using SPHICE: A strongly polarized hydrogen and deuterium ice target

International Nuclear Information System (INIS)

Babusci, D.; Blecher, M.; Breuer, M.; Caracappa, A.; Commeaux, C.; Didelez, J.; Fan, Q.; Giordano, G.; Hicks, K.; Hoblit, S.; Hoffmann-Rothe, P.; Honig, A.; Kistner, O.C.; Khandaker, M.; Li, Z.; Lucas, M.A.; Matone, G.; Miceli, L.; Preedom, B.M.; Rigney, M.; Sandorfi, A.M.; Schaerf, C.; Thorn, C.E.

1995-01-01

Frozen-spin HD polarized targets operating between 0.4 and 4K, used with cold-transfer (4K) techniques, provide great configurational flexibility. Their long depolarization times under target usage conditions assure reasonable match between polarization production and usage times, for weakly ionizing beam fluxes, and the very long relaxation times at fields above 7T (∼1 yr.) provide an economical storage mode and open-quote open-quote off-the-shelf close-quote close-quote availability. copyright 1995 American Institute of Physics

Recent advance in polar seismology: Global impact of the International Polar Year

Science.gov (United States)

Kanao, Masaki; Zhao, Dapeng; Wiens, Douglas A.; Stutzmann, Éléonore

2015-03-01

The most exciting initiative for the recent polar studies was the International Polar Year (IPY) in 2007-2008. The IPY has witnessed a growing community of seismologists who have made considerable efforts to acquire high-quality data in polar regions. It also provided an excellent opportunity to make significant advances in seismic instrumentation of the polar regions to achieve scientific targets involving global issues. Taking these aspects into account, we organize and publish a special issue in Polar Science on the recent advance in polar seismology and cryoseismology as fruitful achievements of the IPY.

Study of excess carrier dynamics in polar, semi-polar, and non-polar (In,Ga)N epilayers and QWs

Energy Technology Data Exchange (ETDEWEB)

Aleksiejunas, R. [Institute of Applied Research, Vilnius University, Sauletekio Ave. 9-III, 10222 Vilnius (Lithuania); Laser Research Center, Vilnius University, Sauletekio Ave. 10, 10222 Vilnius (Lithuania); Lubys, L.; Jarasiunas, K. [Institute of Applied Research, Vilnius University, Sauletekio Ave. 9-III, 10222 Vilnius (Lithuania); Vengris, M. [Laser Research Center, Vilnius University, Sauletekio Ave. 10, 10222 Vilnius (Lithuania); Wernicke, T.; Hoffmann, V.; Netzel, C.; Knauer, A.; Weyers, M. [Ferdinand-Braun-Institut, Leibniz-Institut fuer Hoechstfrequenztechnik, Gustav-Kirchhoff-Str. 4, 12498 Berlin (Germany); Kneissl, M. [Ferdinand-Braun-Institut, Leibniz-Institut fuer Hoechstfrequenztechnik, Gustav-Kirchhoff-Str. 4, 12498 Berlin (Germany); Institute of Solid State Physics, Technische Universitaet Berlin, Hardenbergstr. 36, 10623 Berlin (Germany)

2011-07-15

We studied carrier recombination and diffusion in GaN/sapphire templates, (In,Ga)N layers, and (In,Ga)N quantum well structures oriented along the polar [0001], semi-polar [11-22], and non-polar [11-20] orientations by means of light induced transient grating, differential transmission, and photoluminescence optical techniques. We show that the lifetime of excess carriers drops by orders of magnitude when changing the orientation from polar to non-polar, both in GaN templates and (In,Ga)N layers. We attribute the shorter lifetime to carrier trapping by extended structural defects that are more abundant in non-polar grown samples. In addition, we observe pronounced carrier localization effects in the semi- and non-polar layers. We show that thick (In,Ga)N layers inherit the properties of the GaN templates. However, the thin quantum well structures show a lower carrier trapping activity. So, a better electrical quality can be assumed as compared to the thick (In,Ga)N layers. (copyright 2011 WILEY-VCH Verlag GmbH and Co. KGaA, Weinheim) (orig.)

Polarized targets and beams

International Nuclear Information System (INIS)

Meyer, W.

1985-01-01

First the experimental situation of the single-pion photoproduction and the photodisintegration of the deuteron is briefly discussed. Then a description of the Bonn polarization facilities is given. The point of main effort is put on the polarized target which plays a vital role in the program. A facility for photon induced double polarization experiments at ELSA will be presented in section 4. Properties of a tensor polarized deuteron target are discussed in section 5. The development in the field of polarized targets, especially on new target materials, enables a new generation of polarized target experiments with (polarized) electrons. Some comments on the use of a polarized target in combination with electron beams will be discussed in section 6. Electron deuteron scattering from a tensor polarized deuteron target is considered and compared with other experimental possibilities. (orig./HSI)

Circularly Polarized Luminescence from a Pyrene-Cyclodextrin Supra-Dendron.

Science.gov (United States)

Zhang, Yuening; Yang, Dong; Han, Jianlei; Zhou, Jin; Jin, Qingxian; Liu, Minghua; Duan, Pengfei

2018-05-22

Soft nanomaterials with circularly polarized luminescence (CPL) have been currently attracting great interest. Here, we report a pyrene-containing π-peptide dendron hydrogel, which shows 1D and 2D nanostructures with varied CPL activities. It was found that the individual dendrons formed hydrogels in a wide pH range (3-12) and self-assembled into helices with pH-tuned pitches. Through chirality transfer, the pyrene unit could show CPL originated from both the monomer and excimer bands. When cyclodextrin was introduced, different supra-dendrons were obtained with β-cyclodextrin (PGAc@β-CD) and γ-cyclodextrin (PGAc@γ-CD) through host-guest interactions, respectively. Interestingly, the PGAc@β-CD and PGAc@γ-CD supra-dendrons self-assembled into 2D nanosheet and entangled nanofibers, respectively, showing cyclodextrin induced circularly polarized emission from both the monomer and excimer bands of the pyrene moiety. Thus, through a simple host-guest interaction, both the nanostructures and the chiroptical activities could be modulated.

High-efficiency optical pumping of nuclear polarization in a GaAs quantum well

Science.gov (United States)

Mocek, R. W.; Korenev, V. L.; Bayer, M.; Kotur, M.; Dzhioev, R. I.; Tolmachev, D. O.; Cascio, G.; Kavokin, K. V.; Suter, D.

2017-11-01

The dynamic polarization of nuclear spins by photoexcited electrons is studied in a high quality GaAs/AlGaAs quantum well. We find a surprisingly high efficiency of the spin transfer from the electrons to the nuclei as reflected by a maximum nuclear field of 0.9 T in a tilted external magnetic field of 1 T strength only. This high efficiency is due to a low leakage of spin out of the polarized nuclear system, because mechanisms of spin relaxation other than the hyperfine interaction are strongly suppressed, leading to a long nuclear relaxation time of up to 1000 s. A key ingredient to that end is the low impurity concentration inside the heterostructure, while the electrostatic potential from charged impurities in the surrounding barriers becomes screened through illumination by which the spin relaxation time is increased compared to keeping the system in the dark. This finding indicates a strategy for obtaining high nuclear spin polarization as required for long-lasting carrier spin coherence.

Polarization measurements in high energy elastic scattering of pions, kaons, protons and antiprotons on protons and comparison with Regge phenomenology

International Nuclear Information System (INIS)

Gaidot, A.; Bruneton, C.; Bystricky, J.; Cozzika, G.; Deregel, J.; Ducros, Y.; Khantine-Langlois, F.; Lehar, F.; Lesquen, A. de; Merlo, J.P.; Miyashita, S.; Movchet, J.; Pierrard, J.; Raoul, J.C.; Van Rossum, L.; Kanavets, V.P.

1975-01-01

The polarization parameter P has been measured for elastic scattering on polarized protons, of π - , K - and anti-p at 40GeV/c and of π + , K + and p at 45GeV/c. Four-momentum transfer ranges from -0.08 to -1.8(GeV/c) 2 for π - p and pp, and from -0.08 to -1.2(GeV/c) 2 for π + , K + or K - and anti-p [fr

Effect of 3D Polarization profiles on polarization measurements and colliding beam experiments

Energy Technology Data Exchange (ETDEWEB)

Fischer, W.; Bazilevsky, A.

2011-08-18

The development of polarization profiles are the primary reason for the loss of average polarization. Polarization profiles have been parametrized with a Gaussian distribution. We derive the effect of 3-dimensional polarization profiles on the measured polarization in polarimeters, as well as the observed polarization and the figure of merit in single and double spin experiments. Examples from RHIC are provided. The Relativistic Heavy Ion Collider (RHIC) is the only collider of spin polarized protons. During beam acceleration and storage profiles of the polarization P develop, which affect the polarization measured in a polarimeter, and the polarization and figure of merit (FOM) in colliding beam experiments. We calculate these for profiles in all dimensions, and give examples for RHIC. Like in RHIC we call the two colliding beams Blue and Yellow. We use the overbar to designate intensity-weighted averages in polarimeters (e.g. {bar P}), and angle brackets to designate luminosity-weighted averages in colliding beam experiments (e.g.

).

Effect of 3D Polarization profiles on polarization measurements and colliding beam experiments

International Nuclear Information System (INIS)

Fischer, W.; Bazilevsky, A.

2011-01-01

The development of polarization profiles are the primary reason for the loss of average polarization. Polarization profiles have been parametrized with a Gaussian distribution. We derive the effect of 3-dimensional polarization profiles on the measured polarization in polarimeters, as well as the observed polarization and the figure of merit in single and double spin experiments. Examples from RHIC are provided. The Relativistic Heavy Ion Collider (RHIC) is the only collider of spin polarized protons. During beam acceleration and storage profiles of the polarization P develop, which affect the polarization measured in a polarimeter, and the polarization and figure of merit (FOM) in colliding beam experiments. We calculate these for profiles in all dimensions, and give examples for RHIC. Like in RHIC we call the two colliding beams Blue and Yellow. We use the overbar to designate intensity-weighted averages in polarimeters (e.g. (bar P)), and angle brackets to designate luminosity-weighted averages in colliding beam experiments (e.g. ).

Direct Numerical Simulations of Concentration and Temperature Polarization in Direct Contact Membrane Distillation

Science.gov (United States)

Lou, Jincheng; Tilton, Nils

2017-11-01

Membrane distillation (MD) is a method of desalination with boundary layers that are challenging to simulate. MD is a thermal process in which warm feed and cool distilled water flow on opposite sides of a hydrophobic membrane. The temperature difference causes water to evaporate from the feed, travel through the membrane, and condense in the distillate. Two challenges to MD are temperature and concentration polarization. Temperature polarization represents a reduction in the transmembrane temperature difference due to heat transfer through the membrane. Concentration polarization describes the accumulation of solutes near the membrane. These phenomena reduce filtration and lead to membrane fouling. They are difficult to simulate due to the coupling between the velocity, temperature, and concentration fields on the membrane. Unsteady regimes are particularly challenging because noise at the outlets can pollute the near-membrane flow fields. We present the development of a finite-volume method for the simulation of fluid flow, heat, and mass transport in MD systems. Using the method, we perform a parametric study of the polarization boundary layers, and show that the concentration boundary layer shows self-similar behavior that satisfies power laws for the downstream growth. Funded by the U.S. Bureau of Reclamation.

Nuclear polarization and neutrons

International Nuclear Information System (INIS)

Glaettli, H.

1985-01-01

Different possibilities for the use of polarized nuclei in thermal neutron scattering on condensed matter are reviewed. Highly polarized nuclei are the starting point for studying dipolar magnetic order. Systematic measurement of spin-dependent scattering lengths is possible on samples with polarized nuclei. Highly polarized hydrogen should help to unravel complicated structures in chemistry and biology. The use of polarized proton targets as an energy-independent neutron polarizer in the thermal and epithermal region should be considered afresh. (author)

The Hanle and Zeeman Polarization Signals of the Solar Ca II 8542 angstromLine

Czech Academy of Sciences Publication Activity Database

Štěpán, Jiří; Trujillo Bueno, J.

2016-01-01

Roč. 826, č. 1 (2016), L10/1-L10/6 ISSN 2041-8205 R&D Projects: GA ČR(CZ) GA16-16861S Grant - others:COST Action(XE) MP1104 Institutional support: RVO:67985815 Keywords : line profiles * polarization * radiative transfer Subject RIV: BN - Astronomy, Celestial Mechanics, Astrophysics Impact factor: 5.522, year: 2016

Convective mass transfer in helical pipes: effect of curvature and torsion

Energy Technology Data Exchange (ETDEWEB)

Litster, S.; Djilali, N. [University of Victoria, Department of Mechanical Engineering, Victoria, BC (Canada); Pharoah, J.G. [University of Victoria, Department of Mechanical Engineering, Victoria, BC (Canada); Queen' s University at Kingston, Department of Mechanical Engineering, Kingston, ON (Canada)

2006-03-01

A 3D numerical analysis of the flow and mass transfer in helical pipes is presented. The interpretation of the flow patterns and their impact on mass transfer is shown to require a non-orthogonal pseudo-stream function based visualization. The strong coupling between torsion and curvature effects, and the resulting secondary flow regimes are well characterized by a parameter combining both the Dean (Dn) and Germano numbers (Gn). For membrane separation applications, helical modules combining high curvature with low torsion would alleviate concentration polarization and yield appreciable flux improvement. (orig.)

Kinetic isotope effects and tunnelling in the proton-transfer reaction between 4-nitrophenylnitromethane and tetramethylguanidine in various aprotic solvents

International Nuclear Information System (INIS)

Caldin, E.F.; Mateo, S.

1975-01-01

Rates and equilibrium constants have been determined for the proton-transfer reaction of 4-nitrophenylnitromethane, NO 2 C 6 H 4 CH 2 NO 2 , and its αα-deuterated analogue NO 2 C 6 H 4 CD 2 NO 2 , with the strong base tetramethylguanidine [HN=C(NMe 2 ) 2 ), at temperatures between -60 0 C and +65 0 in a range of aprotic solvents. Spectrophotometry and the stopped-flow technique were used. The reaction is a simple proton-transfer process leading to an ion-pair. The kinetic isotope effects are correlated with the polarity of the solvents, as measured by the dielectric constant or by the empirical parameter Esub(T). In the less polar solvents they are exceptionally large. In toluene, for example, at 25 0 C the rate ratio ksup(H)/ksup(D) = 45 +- 2, the activation energy difference Esub(a)sup(D) - Esub(a)sup(H) =4.3 +- 0.3 kcal molsup(-1) (16 kJ molsup(-1), and the ratio of the pre-exponential factors logsub(10) (Asup(D)/Asup(H)) = 1.5 +- 0.2+ and even larger values of logsub(10)(Asup(D)/Asup(H)) are found for mesitylene (1.94 +- 0.06) and cyclohexane (2.4 +- 0.2). Positive deviations from linear Arrhenius plots are found for these solvents. Tunnelling is the only interpretation that cannot account for these results. For the more polar solvents (dielectric constant 7 to 37), the isotope effects are closer to the range predicted by semi-classical theory. The isotope effects in all solvents have been fitted to Bell's equation for a parabolic barrier, and the barrier dimensions calculated for each solvent. The suggested interpretation of the results is that the solvent-solute interactions affect the height of the barrier and that motions of solvent molecules are coupled with the motion of the proton in the more polar solvents but not in the less polar ones; reorganization of solvent molecules accompanies the proton-transfer in the more polar solvents, but only electron-polarization in the less polar. Tunnelling has large effects in the less polar solvents, where the

NUCLEON POLARIZATION IN 3-BODY MODELS OF POLARIZED LI-6

NARCIS (Netherlands)

SCHELLINGERHOUT, NW; KOK, LP; COON, SA; ADAM, RM

1993-01-01

Just as He-3 --> can be approximately characterized as a polarized neutron target, polarized Li-6D has been advocated as a good isoscalar nuclear target for the extraction of the polarized gluon content of the nucleon. The original argument rests upon a presumed ''alpha + deuteron'' picture of Li-6,

Superconducting polarizing magnet for a movable polarized target

International Nuclear Information System (INIS)

Anishchenko, N.G.; Bartenev, V.D.; Blinov, N.A.

1998-01-01

The superconducting polarizing magnet was constructed for the JINR (Dubna) movable polarized target (MPT) with working volume 200 mm long and 30 mm in diameter. The magnet provides a polarizing magnetic field up to 6 T in the centre with the uniformity of 4.5 x 10 -4 in the working volume of the target. The magnet contains a main solenoidal winding 558 mm long and 206/144 mm in diameters, and compensating and correcting winding placed at its ends. The windings are made of a NbTi wire, impregnated with the epoxy resin and placed in the horizontal cryostat. The diameter of the 'warm' aperture of the magnet cryostat is 96 mm. The design and technology of the magnet winding are described. Results of the magnetic field map measurements, using a NMR-magnetometer are given. A similar magnet constructed at DAPNIA, CEA/Saclay (France), represented a model for the present development. The MPT array is installed in the beam line of polarized neutrons produced by break-up of polarized deuterons extracted from the synchrophasotron of the Laboratory of High Energies (LHE), JINR (Dubna)

How to learn about polarized lambda-baryon fragmentation functions?

International Nuclear Information System (INIS)

Soffer, J.

1999-01-01

We study the inclusive production of Λ (Λ-bar) in several high energy collision processes (e + e - , e ± p, ν(ν-bar)p, pp), in view of an accurate determination of the polarized fragmentation functions of a quark into a Λ (Λ-bar). We will recall that present data are unable to distinguish between various theoretical models, in particular for the spin transfer mechanisms and we will indicate how future measurements will provide ways to discriminate between them and also how to achieve a necessary quark flavor separation

Polarization observables in deuteron photodisintegration below 360 MeV

International Nuclear Information System (INIS)

2011-01-01

High precision measurements of induced and transferred recoil proton polarization in d((rvec y), (rvec p))n have been performed for photon energies of 277-357 MeV and θcm = 20 o -120 o . The measurements were motivated by a longstanding discrepancy between meson-baryon model calculations and data at higher energies. At the low energies of this experiment, theory continues to fail to reproduce the data, indicating that either something is missing in the calculations and/or there is a problem with the accuracy of the nucleon-nucleon potential being used.

Polarization observables in deuteron photodisintegration below 360 MeV

Science.gov (United States)

Glister, J.; Ron, G.; Lee, B. W.; Gilman, R.; Sarty, A. J.; Strauch, S.; Higinbotham, D. W.; Piasetzky, E.; Allada, K.; Armstrong, W.; Arrington, J.; Arenhövel, H.; Beck, A.; Benmokhtar, F.; Berman, B. L.; Boeglin, W.; Brash, E.; Camsonne, A.; Calarco, J.; Chen, J. P.; Choi, S.; Chudakov, E.; Coman, L.; Craver, B.; Cusanno, F.; Dumas, J.; Dutta, C.; Feuerbach, R.; Freyberger, A.; Frullani, S.; Garibaldi, F.; Hansen, J.-O.; Holmstrom, T.; Hyde, C. E.; Ibrahim, H.; Ilieva, Y.; de Jager, C. W.; Jiang, X.; Jones, M. K.; Kang, Hyekoo; Kelleher, A.; Khrosinkova, E.; Kuchina, E.; Kumbartzki, G.; LeRose, J. J.; Lindgren, R.; Markowitz, P.; May-Tal Beck, S.; McCullough, E.; Meekins, D.; Meziane, M.; Meziani, Z.-E.; Michaels, R.; Moffit, B.; Norum, B. E.; Oh, Y.; Olson, M.; Paolone, M.; Paschke, K.; Perdrisat, C. F.; Potokar, M.; Pomatsalyuk, R.; Pomerantz, I.; Puckett, A.; Punjabi, V.; Qian, X.; Qiang, Y.; Ransome, R. D.; Reyhan, M.; Roche, J.; Rousseau, Y.; Saha, A.; Sawatzky, B.; Schulte, E.; Schwamb, M.; Shabestari, M.; Shahinyan, A.; Shneor, R.; Širca, S.; Slifer, K.; Solvignon, P.; Song, J.; Sparks, R.; Subedi, R.; Urciuoli, G. M.; Wang, K.; Wojtsekhowski, B.; Yan, X.; Yao, H.; Zhan, X.; Zhu, X.

2011-03-01

High precision measurements of induced and transferred recoil proton polarization in d(γ→,p→)n have been performed for photon energies of 277-357 MeV and θcm=20°-120°. The measurements were motivated by a longstanding discrepancy between meson-baryon model calculations and data at higher energies. At the low energies of this experiment, theory continues to fail to reproduce the data, indicating that either something is missing in the calculations and/or there is a problem with the accuracy of the nucleon-nucleon potential being used.

CMB polarization at large angular scales: Data analysis of the POLAR experiment

International Nuclear Information System (INIS)

O'Dell, Christopher W.; Keating, Brian G.; Oliveira-Costa, Angelica de; Tegmark, Max; Timbie, Peter T.

2003-01-01

The coming flood of cosmic microwave background (CMB) polarization experiments, spurred by the recent detection of CMB polarization by the DASI and WMAP instruments, will be confronted by many new analysis tasks specific to polarization. For the analysis of CMB polarization data sets, the devil is truly in the details. With this in mind, we present details of the data analysis for the POLAR experiment, which recently led to the tightest upper limits on the polarization of the cosmic microwave background radiation at large angular scales. We discuss the data selection process, map-making algorithms, offset removal, and likelihood analysis which were used to find upper limits on the polarization. Stated using the modern convention for reporting CMB Stokes parameters, these limits are 5.0 μK on both E- and B-type polarization at 95% confidence. Finally, we discuss simulations used to test our analysis techniques and to probe the fundamental limitations of the experiment

Solvent effects on the excited-state double proton transfer mechanism in the 7-azaindole dimer: a TDDFT study with the polarizable continuum model.

Science.gov (United States)

Yu, Xue-Fang; Yamazaki, Shohei; Taketsugu, Tetsuya

2017-08-30

Solvent effects on the excited-state double proton transfer (ESDPT) mechanism in the 7-azaindole (7AI) dimer were investigated using the time-dependent density functional theory (TDDFT) method. Excited-state potential energy profiles along the reaction paths in a locally excited (LE) state and a charge transfer (CT) state were calculated using the polarizable continuum model (PCM) to include the solvent effect. A series of non-polar and polar solvents with different dielectric constants were used to examine the polarity effect on the ESDPT mechanism. The present results suggest that in a non-polar solvent and a polar solvent with a small dielectric constant, ESDPT follows a concerted mechanism, similar to the case in the gas phase. In a polar solvent with a relatively large dielectric constant, however, ESDPT is likely to follow a stepwise mechanism via a stable zwitterionic intermediate in the LE state on the adiabatic potential energy surface, although inclusion of zero-point vibrational energy (ZPE) corrections again suggests the concerted mechanism. In the meantime, the stepwise reaction path involving the CT state with neutral intermediates is also examined, and is found to be less competitive than the concerted or stepwise path in the LE state in both non-polar and polar solvents. The present study provides a new insight into the experimental controversy of the ESDPT mechanism of the 7AI dimer in a solution.

Chemical nuclear polarization effects in photoreactions of 1,4-diazabicyclo[2.2.2]octane with carbonyl-containing compounds

Science.gov (United States)

Porkhun, V. I.; Rakhimov, A. I.

2012-11-01

Elementary acts of the photoreaction of diamine with 2,6-diphenyl- p-benzoquinone are determined from the effects of chemical nuclear polarization effects. Hydrogen atom transfer is shown to occur in two stages with the participation of a radical ion pair.

Climate impact of idealized winter polar mesospheric and stratospheric ozone losses as caused by energetic particle precipitation

Directory of Open Access Journals (Sweden)

K. Meraner

2018-01-01

Full Text Available Energetic particles enter the polar atmosphere and enhance the production of nitrogen oxides and hydrogen oxides in the winter stratosphere and mesosphere. Both components are powerful ozone destroyers. Recently, it has been inferred from observations that the direct effect of energetic particle precipitation (EPP causes significant long-term mesospheric ozone variability. Satellites observe a decrease in mesospheric ozone up to 34 % between EPP maximum and EPP minimum. Stratospheric ozone decreases due to the indirect effect of EPP by about 10–15 % observed by satellite instruments. Here, we analyze the climate impact of winter boreal idealized polar mesospheric and polar stratospheric ozone losses as caused by EPP in the coupled Max Planck Institute Earth System Model (MPI-ESM. Using radiative transfer modeling, we find that the radiative forcing of mesospheric ozone loss during polar night is small. Hence, climate effects of mesospheric ozone loss due to energetic particles seem unlikely. Stratospheric ozone loss due to energetic particles warms the winter polar stratosphere and subsequently weakens the polar vortex. However, those changes are small, and few statistically significant changes in surface climate are found.

Transfer function and near-field detection of evanescent waves

DEFF Research Database (Denmark)

Radko, Ylia P.; Bozhevolnyi, Sergey I.; Gregersen, Niels

2006-01-01

of collection and illumination modes. Making use of a collection near-field microscope with a similar fiber tip illuminated by an evanescent field, we measure the collected power as a function of the field spatial frequency in different polarization configurations. Considering a two-dimensional probe...... for the transfer function, which is derived by introducing an effective pointof (dipolelike) detection inside the probe tip. It is found to be possible to fit reasonably well both the experimental and the simulation data for evanescent field components, implying that the developed approximation of the near......-field transfer function can serve as a simple, rational, and sufficiently reliable means of fiber probe characterization....

Energy and polarization dependence of resonant inelastic X-ray scattering in Nd2CuO4

International Nuclear Information System (INIS)

Hill, J.P.; Kao, C.C.; Haemaelaeinen, K.

1998-01-01

The authors report the energy and polarization dependence of resonant inelastic x-ray scattering from Nd 2 CuO 4 . An energy loss feature at ∼6 eV is observed in the vicinity of the Cu K-edge. Numerical calculations based on the Anderson impurity model identify this as a charge transfer excitation to the anti-bonding state. The incident polarization is shown to select the intermediate states participating in the resonance process. Resonances are observed at 8,990 eV and 9,000 eV with the incident polarization perpendicular and parallel to the CuO planes, respectively. In contrast to the single-site model calculations, no resonances are observed associated with the 1s3d 10 L intermediate states, suggesting non-local effects play a role

Few-body experiments with polarized beams and polarized targets

International Nuclear Information System (INIS)

Simmons, J.E.

1983-01-01

A survey is presented concerning recent polarization experiments in the elastic p-d, p- 3 He, and p- 4 He systems. Mention is made of selected neutron experiments. The nominal energy range is 10 to 1000 MeV. Recent results and interpretations of the p-d system near 10 MeV are discussed. New experiments on the energy dependence of back angle p-d tensor polarization are discussed with respect to resolution of discrepancies and difficulty of theoretical interpretation. Progress is noted concerning multiple scattering interpretation of forward p-d deuteron polarization. Some new results are presented concerning the p- 3 He system and higher energy p- 4 He polarization experiments. 52 references

NMR study of hyper-polarized 129Xe and applications to liquid-phase NMR experiments

International Nuclear Information System (INIS)

Marion, D.

2008-07-01

In liquid samples where both nuclear polarization and spin density are strong, the magnetization dynamics, which can be analysed by NMR (nuclear magnetic resonance) methods, is deeply influenced by the internal couplings induced by local dipolar fields. The present thesis describes some of the many consequences associated to the presence in the sample of concentrated xenon hyper-polarized by an optical pumping process. First, we deal with the induced modifications in frequency and line width of the proton and xenon spectra, then we present the results of SPIDER, a coherent polarization transfer experiment designed to enhance the polarization of protons, in order to increase their NMR signal level. A third part is dedicated to the description of the apparition of repeated chaotic maser emissions by un unstable xenon magnetization coupled to the detection coil tuned at the xenon Larmor frequency (here 138 MHz). In the last part, we present a new method allowing a better tuning of any NMR detection probe and resulting in sensible gains in terms of sensitivity and signal shaping. Finally, we conclude with a partial questioning of the classical relaxation theory in the specific field of highly polarized and concentrated spin systems in a liquid phase. (author)

Marine foraging and annual fish consumption of a south polar Skua population in the maritime Antarctic

NARCIS (Netherlands)

Hahn, S.M.; Ritz, M.S.; Reinhardt, K.

2008-01-01

Pelagic fish are an important component of Antarctic food webs but few quantitative data exist on energy transfer from fish to seabirds for the Seasonal Pack-ice Zone. We studied a local population of south polar, skuas Catharacta maccormicki during a whole breeding cycle and estimated its entire

Long-period polar rain variations, solar wind and hemispherically symmetric polar rain

International Nuclear Information System (INIS)

Makita, K.; Meng, C.

1987-01-01

On the basic of electron data obtained by the Defense Meteorological Satellite Program (DMSP) F2 satellite the long-period variations of the polar rain flux are examined for four consecutive solar rotations. It is clearly demonstrated that the asymmetric enhancement of the polar rain flux is strongly controlled by the sector structure of the interplanetary magnetic field (IMF). However, the orbit-to-orbit and day-to-day variations of the polar rain flux are detected even during a very stable sector period, and the polar rain flux does not have any clear relationship to the magnitude of the IMF B/sub x/ or B/sub y/. Thus the polarity of B/sub x/ controls only the accessibility of a polar region. It is also noticed that the intensity of polar rain fluxes does not show any relationship to the density of the solar wind, suggesting that the origin of the polar rain electrons is different from the commonly observed part of the solar wind electron distribution function. In addition to the asymmetric polar rain distribution, increasing polar rain fluxes of similar high intensity are sometimes detected over both polar caps. An examination of more than 1 year's data from the DMSP F2 and F4 satellites shows that simultaneous intense uniform precipitations (>10 7 electrons/cm 2 s sr) over both polar caps are not coincidental; it also shows that the spectra are similar. The occurrence of hemispherically symmetric events is not common. They generally are observed after an IMF sector transition period, during unstable periods in the sector structure, and while the solar wind density is high. copyright American Geophysical Union 1987

Polarized Radiative Transfer of a Cirrus Cloud Consisting of Randomly Oriented Hexagonal Ice Crystals: The 3 x 3 Approximation for Non-Spherical Particles

Science.gov (United States)

Stamnes, S.; Ou, S. C.; Lin, Z.; Takano, Y.; Tsay, S. C.; Liou, K.N.; Stamnes, K.

2016-01-01

The reflection and transmission of polarized light for a cirrus cloud consisting of randomly oriented hexagonal columns were calculated by two very different vector radiative transfer models. The forward peak of the phase function for the ensemble-averaged ice crystals has a value of order 6 x 10(exp 3) so a truncation procedure was used to help produce numerically efficient yet accurate results. One of these models, the Vectorized Line-by-Line Equivalent model (VLBLE), is based on the doubling- adding principle, while the other is based on a vector discrete ordinates method (VDISORT). A comparison shows that the two models provide very close although not entirely identical results, which can be explained by differences in treatment of single scattering and the representation of the scattering phase matrix. The relative differences in the reflected I and Q Stokes parameters are within 0.5 for I and within 1.5 for Q for all viewing angles. In 1971 Hansen showed that for scattering by spherical particles the 3 x 3 approximation is sufficient to produce accurate results for the reflected radiance I and the degree of polarization (DOP), and he conjectured that these results would hold also for non-spherical particles. Simulations were conducted to test Hansen's conjecture for the cirrus cloud particles considered in this study. It was found that the 3 x 3 approximation also gives accurate results for the transmitted light, and for Q and U in addition to I and DOP. For these non-spherical ice particles the 3 x 3 approximation leads to an absolute error 2 x 10(exp -6) for the reflected and transmitted I, Q and U Stokes parameters. Hence, it appears to be an excellent approximation, which significantly reduces the computational complexity and burden required for multiple scattering calculations.

Degree of polarization and source counts of faint radio sources from Stacking Polarized intensity

International Nuclear Information System (INIS)

Stil, J. M.; George, S. J.; Keller, B. W.; Taylor, A. R.

2014-01-01

We present stacking polarized intensity as a means to study the polarization of sources that are too faint to be detected individually in surveys of polarized radio sources. Stacking offers not only high sensitivity to the median signal of a class of radio sources, but also avoids a detection threshold in polarized intensity, and therefore an arbitrary exclusion of sources with a low percentage of polarization. Correction for polarization bias is done through a Monte Carlo analysis and tested on a simulated survey. We show that the nonlinear relation between the real polarized signal and the detected signal requires knowledge of the shape of the distribution of fractional polarization, which we constrain using the ratio of the upper quartile to the lower quartile of the distribution of stacked polarized intensities. Stacking polarized intensity for NRAO VLA Sky Survey (NVSS) sources down to the detection limit in Stokes I, we find a gradual increase in median fractional polarization that is consistent with a trend that was noticed before for bright NVSS sources, but is much more gradual than found by previous deep surveys of radio polarization. Consequently, the polarized radio source counts derived from our stacking experiment predict fewer polarized radio sources for future surveys with the Square Kilometre Array and its pathfinders.

Polarization developments

International Nuclear Information System (INIS)

Prescott, C.Y.

1993-07-01

Recent developments in laser-driven photoemission sources of polarized electrons have made prospects for highly polarized electron beams in a future linear collider very promising. This talk discusses the experiences with the SLC polarized electron source, the recent progress with research into gallium arsenide and strained gallium arsenide as a photocathode material, and the suitability of these cathode materials for a future linear collider based on the parameters of the several linear collider designs that exist

Time-resolved stimulated emission depletion and energy transfer dynamics in two-photon excited EGFP

Science.gov (United States)

Masters, T. A.; Robinson, N. A.; Marsh, R. J.; Blacker, T. S.; Armoogum, D. A.; Larijani, B.; Bain, A. J.

2018-04-01

Time and polarization-resolved stimulated emission depletion (STED) measurements are used to investigate excited state evolution following the two-photon excitation of enhanced green fluorescent protein (EGFP). We employ a new approach for the accurate STED measurement of the hitherto unmeasured degree of hexadecapolar transition dipole moment alignment ⟨α40 ⟩ present at a given excitation-depletion (pump-dump) pulse separation. Time-resolved polarized fluorescence measurements as a function of pump-dump delay reveal the time evolution of ⟨α40 ⟩ to be considerably more rapid than predicted for isotropic rotational diffusion in EGFP. Additional depolarization by homo-Förster resonance energy transfer is investigated for both ⟨α20 ⟩ (quadrupolar) and ⟨α40 ⟩ transition dipole alignments. These results point to the utility of higher order dipole correlation measurements in the investigation of resonance energy transfer processes.

Geographical Income Polarization

DEFF Research Database (Denmark)

Azhar, Hussain; Jonassen, Anders Bruun

inter municipal income inequality. Counter factual simulations show that rising property prices to a large part explain the rise in polarization. One side-effect of polarization is tendencies towards a parallel polarization of residence location patterns, where low skilled individuals tend to live...

Perceiving polarization with the naked eye: characterization of human polarization sensitivity

Science.gov (United States)

Temple, Shelby E.; McGregor, Juliette E.; Miles, Camilla; Graham, Laura; Miller, Josie; Buck, Jordan; Scott-Samuel, Nicholas E.; Roberts, Nicholas W.

2015-01-01

Like many animals, humans are sensitive to the polarization of light. We can detect the angle of polarization using an entoptic phenomenon called Haidinger's brushes, which is mediated by dichroic carotenoids in the macula lutea. While previous studies have characterized the spectral sensitivity of Haidinger's brushes, other aspects remain unexplored. We developed a novel methodology for presenting gratings in polarization-only contrast at varying degrees of polarization in order to measure the lower limits of human polarized light detection. Participants were, on average, able to perform the task down to a threshold of 56%, with some able to go as low as 23%. This makes humans the most sensitive vertebrate tested to date. Additionally, we quantified a nonlinear relationship between presented and perceived polarization angle when an observer is presented with a rotatable polarized light field. This result confirms a previous theoretical prediction of how uniaxial corneal birefringence impacts the perception of Haidinger's brushes. The rotational dynamics of Haidinger's brushes were then used to calculate corneal retardance. We suggest that psychophysical experiments, based upon the perception of polarized light, are amenable to the production of affordable technologies for self-assessment and longitudinal monitoring of visual dysfunctions such as age-related macular degeneration. PMID:26136441

Polarization and charge transfer in the hydration of chloride ions

International Nuclear Information System (INIS)

Zhao Zhen; Rogers, David M.; Beck, Thomas L.

2010-01-01

A theoretical study of the structural and electronic properties of the chloride ion and water molecules in the first hydration shell is presented. The calculations are performed on an ensemble of configurations obtained from molecular dynamics simulations of a single chloride ion in bulk water. The simulations utilize the polarizable AMOEBA force field for trajectory generation and MP2-level calculations are performed to examine the electronic structure properties of the ions and surrounding waters in the external field of more distant waters. The ChelpG method is employed to explore the effective charges and dipoles on the chloride ions and first-shell waters. The quantum theory of atoms in molecules (QTAIM) is further utilized to examine charge transfer from the anion to surrounding water molecules. The clusters extracted from the AMOEBA simulations exhibit high probabilities of anisotropic solvation for chloride ions in bulk water. From the QTAIM analysis, 0.2 elementary charges are transferred from the ion to the first-shell water molecules. The default AMOEBA model overestimates the average dipole moment magnitude of the ion compared to the quantum mechanical value. The average magnitude of the dipole moment of the water molecules in the first shell treated at the MP2-level, with the more distant waters handled with an AMOEBA effective charge model, is 2.67 D. This value is close to the AMOEBA result for first-shell waters (2.72 D) and is slightly reduced from the bulk AMOEBA value (2.78 D). The magnitude of the dipole moment of the water molecules in the first solvation shell is most strongly affected by the local water-water interactions and hydrogen bonds with the second solvation shell, rather than by interactions with the ion.

Iterative atmospheric correction scheme and the polarization color of alpine snow

Science.gov (United States)

Ottaviani, Matteo; Cairns, Brian; Ferrare, Rich; Rogers, Raymond

2012-07-01

Characterization of the Earth's surface is crucial to remote sensing, both to map geomorphological features and because subtracting this signal is essential during retrievals of the atmospheric constituents located between the surface and the sensor. Current operational algorithms model the surface total reflectance through a weighted linear combination of a few geometry-dependent kernels, each devised to describe a particular scattering mechanism. The information content of these measurements is overwhelmed by that of instruments with polarization capabilities: proposed models in this case are based on the Fresnel reflectance of an isotropic distribution of facets. Because of its remarkable lack of spectral contrast, the polarized reflectance of land surfaces in the shortwave infrared spectral region, where atmospheric scattering is minimal, can be used to model the surface also at shorter wavelengths, where aerosol retrievals are attempted based on well-established scattering theories.In radiative transfer simulations, straightforward separation of the surface and atmospheric contributions is not possible without approximations because of the coupling introduced by multiple reflections. Within a general inversion framework, the problem can be eliminated by linearizing the radiative transfer calculation, and making the Jacobian (i.e., the derivative expressing the sensitivity of the reflectance with respect to model parameters) available at output. We present a general methodology based on a Gauss-Newton iterative search, which automates this procedure and eliminates de facto the need of an ad hoc atmospheric correction.In this case study we analyze the color variations in the polarized reflectance measured by the NASA Goddard Institute of Space Studies Research Scanning Polarimeter during a survey of late-season snowfields in the High Sierra. This insofar unique dataset presents challenges linked to the rugged topography associated with the alpine environment and

Iterative atmospheric correction scheme and the polarization color of alpine snow

International Nuclear Information System (INIS)

Ottaviani, Matteo; Cairns, Brian; Ferrare, Rich; Rogers, Raymond

2012-01-01

Characterization of the Earth's surface is crucial to remote sensing, both to map geomorphological features and because subtracting this signal is essential during retrievals of the atmospheric constituents located between the surface and the sensor. Current operational algorithms model the surface total reflectance through a weighted linear combination of a few geometry-dependent kernels, each devised to describe a particular scattering mechanism. The information content of these measurements is overwhelmed by that of instruments with polarization capabilities: proposed models in this case are based on the Fresnel reflectance of an isotropic distribution of facets. Because of its remarkable lack of spectral contrast, the polarized reflectance of land surfaces in the shortwave infrared spectral region, where atmospheric scattering is minimal, can be used to model the surface also at shorter wavelengths, where aerosol retrievals are attempted based on well-established scattering theories. In radiative transfer simulations, straightforward separation of the surface and atmospheric contributions is not possible without approximations because of the coupling introduced by multiple reflections. Within a general inversion framework, the problem can be eliminated by linearizing the radiative transfer calculation, and making the Jacobian (i.e., the derivative expressing the sensitivity of the reflectance with respect to model parameters) available at output. We present a general methodology based on a Gauss-Newton iterative search, which automates this procedure and eliminates de facto the need of an ad hoc atmospheric correction. In this case study we analyze the color variations in the polarized reflectance measured by the NASA Goddard Institute of Space Studies Research Scanning Polarimeter during a survey of late-season snowfields in the High Sierra. This insofar unique dataset presents challenges linked to the rugged topography associated with the alpine environment

Measurement of the polarized neutron---polarized 3He total cross section

International Nuclear Information System (INIS)

Keith, C.D.; Gould, C.R.; Haase, D.G.; Seely, M.L.; Huffman, P.R.; Roberson, N.R.; Tornow, W.; Wilburn, W.S.

1995-01-01

The first measurements of polarized neutron--polarized 3 He scattering in the few MeV energy region are reported. The total cross section difference Δσ T for transversely polarized target and beam has been measured for neutron energies between 1.9 and 7.5 MeV. Comparison is made to predictions of Δσ T using various descriptions of the 4 He continuum. A brute-force polarized target of solid 3 He has been developed for these measurements. The target is 4.3x10 22 atoms/cm 2 thick and is polarized to 38% at 7 Telsa and 12 mK. copyright 1995 American Institute of Physics

Scattering with polarized neutrons

International Nuclear Information System (INIS)

Schweizer, J.

2007-01-01

In the history of neutron scattering, it was shown very soon that the use of polarized neutron beams brings much more information than usual scattering with unpolarized neutrons. We shall develop here the different scattering methods that imply polarized neutrons: 1) polarized beams without polarization analysis, the flipping ratio method; 2) polarized beams with a uniaxial polarization analysis; 3) polarized beams with a spherical polarization analysis. For all these scattering methods, we shall give examples of the physical problems which can been solved by these methods, particularly in the field of magnetism: investigation of complex magnetic structures, investigation of spin or magnetization densities in metals, insulators and molecular compounds, separation of magnetic and nuclear scattering, investigation of magnetic properties of liquids and amorphous materials and even, for non magnetic material, separation between coherent and incoherent scattering. (author)

Low-temperature dynamic nuclear polarization at 9.4 T with a 30 mW microwave source.

Science.gov (United States)

Thurber, Kent R; Yau, Wai-Ming; Tycko, Robert

2010-06-01

Dynamic nuclear polarization (DNP) can provide large signal enhancements in nuclear magnetic resonance (NMR) by transfer of polarization from electron spins to nuclear spins. We discuss several aspects of DNP experiments at 9.4 T (400 MHz resonant frequency for (1)H, 264 GHz for electron spins in organic radicals) in the 7-80K temperature range, using a 30 mW, frequency-tunable microwave source and a quasi-optical microwave bridge for polarization control and low-loss microwave transmission. In experiments on frozen glycerol/water doped with nitroxide radicals, DNP signal enhancements up to a factor of 80 are observed (relative to (1)H NMR signals with thermal equilibrium spin polarization). The largest sensitivity enhancements are observed with a new triradical dopant, DOTOPA-TEMPO. Field modulation with a 10 G root-mean-squared amplitude during DNP increases the nuclear spin polarizations by up to 135%. Dependencies of (1)H NMR signal amplitudes, nuclear spin relaxation times, and DNP build-up times on the dopant and its concentration, temperature, microwave power, and modulation frequency are reported and discussed. The benefits of low-temperature DNP can be dramatic: the (1)H spin polarization is increased approximately 1000-fold at 7 K with DNP, relative to thermal polarization at 80K. (c) 2010 Elsevier Inc. All rights reserved.

Dynamically polarized hydrogen target as a broadband, wavelength-independent thermal neutron spin polarizer

International Nuclear Information System (INIS)

Zhao Jinkui; Garamus, Vasil M.; Mueller, Wilhelm; Willumeit, Regine

2005-01-01

A hydrogen-rich sample with dynamically polarized hydrogen nuclei was tested as a wavelength-independent neutron transmission spin polarizer. The experiment used a modified setup of the dynamic nuclear polarization target station at the GKSS research center. The standard solvent sample at the GKSS DNP station was used. It is 2.8mm thick and consists of 43.4wt% water, 54.6wt% glycerol, and 2wt% of EHBA-Cr(v) complex. The wavelength of the incident neutrons for the transmission experiment was λ=8.1A with Δλ/λ=10%. The polarization of neutron beam after the target sample was analyzed with a supermirror analyzer. A neutron polarization of -52% was achieved at the hydrogen polarization of -69%. Further experiments will test the feasibility of other hydrogen-rich materials, such as methane, as the polarizer. A theoretical calculation shows that a polarized methane target would allow over 95% neutron polarizations with more than 30% transmission