The relative impact of photoionizing radiation and stellar winds on different environments
Haid, S.; Walch, S.; Seifried, D.; Wünsch, R.; Dinnbier, F.; Naab, T.
2018-05-01
Photoionizing radiation and stellar winds from massive stars deposit energy and momentum into the interstellar medium (ISM). They might disperse the local ISM, change its turbulent multi-phase structure, and even regulate star formation. Ionizing radiation dominates the massive stars' energy output, but the relative effect of winds might change with stellar mass and the properties of the ambient ISM. We present simulations of the interaction of stellar winds and ionizing radiation of 12, 23, and 60 M⊙ stars within a cold neutral (CNM, n0 = 100 cm-3), warm neutral (WNM, n0 = 1, 10 cm-3) or warm ionized (WIM, n0 = 0.1 cm-3) medium. The FLASH simulations adopt the novel tree-based radiation transfer algorithm TREERAY. With the On-the-Spot approximation and a temperature-dependent recombination coefficient, it is coupled to a chemical network with radiative heating and cooling. In the homogeneous CNM, the total momentum injection ranges from 1.6× 104 to 4× 105 M⊙ km s-1 and is always dominated by the expansion of the ionized HII region. In the WIM, stellar winds dominate (2× 102 to 5× 103 M⊙ km s-1), while the input from radiation is small (˜ 102 M⊙ km s-1). The WNM (n0 = 1 cm-3) is a transition regime. Energetically, stellar winds couple more efficiently to the ISM (˜ 0.1 percent of wind luminosity) than radiation (< 0.001 percent of ionizing luminosity). For estimating the impact of massive stars, the strongly mass-dependent ratios of wind to ionizing luminosity and the properties of the ambient medium have to be considered.
AXISYMMETRIC SIMULATIONS OF HOT JUPITER–STELLAR WIND HYDRODYNAMIC INTERACTION
International Nuclear Information System (INIS)
Christie, Duncan; Arras, Phil; Li, Zhi-Yun
2016-01-01
Gas giant exoplanets orbiting at close distances to the parent star are subjected to large radiation and stellar wind fluxes. In this paper, hydrodynamic simulations of the planetary upper atmosphere and its interaction with the stellar wind are carried out to understand the possible flow regimes and how they affect the Lyα transmission spectrum. Following Tremblin and Chiang, charge exchange reactions are included to explore the role of energetic atoms as compared to thermal particles. In order to understand the role of the tail as compared to the leading edge of the planetary gas, the simulations were carried out under axisymmetry, and photoionization and stellar wind electron impact ionization reactions were included to limit the extent of the neutrals away from the planet. By varying the planetary gas temperature, two regimes are found. At high temperature, a supersonic planetary wind is found, which is turned around by the stellar wind and forms a tail behind the planet. At lower temperatures, the planetary wind is shut off when the stellar wind penetrates inside where the sonic point would have been. In this regime mass is lost by viscous interaction at the boundary between planetary and stellar wind gases. Absorption by cold hydrogen atoms is large near the planetary surface, and decreases away from the planet as expected. The hot hydrogen absorption is in an annulus and typically dominated by the tail, at large impact parameter, rather than by the thin leading edge of the mixing layer near the substellar point
AXISYMMETRIC SIMULATIONS OF HOT JUPITER–STELLAR WIND HYDRODYNAMIC INTERACTION
Energy Technology Data Exchange (ETDEWEB)
Christie, Duncan; Arras, Phil; Li, Zhi-Yun [Department of Astronomy, University of Virginia, Charlottesville, VA 22904 (United States)
2016-03-20
Gas giant exoplanets orbiting at close distances to the parent star are subjected to large radiation and stellar wind fluxes. In this paper, hydrodynamic simulations of the planetary upper atmosphere and its interaction with the stellar wind are carried out to understand the possible flow regimes and how they affect the Lyα transmission spectrum. Following Tremblin and Chiang, charge exchange reactions are included to explore the role of energetic atoms as compared to thermal particles. In order to understand the role of the tail as compared to the leading edge of the planetary gas, the simulations were carried out under axisymmetry, and photoionization and stellar wind electron impact ionization reactions were included to limit the extent of the neutrals away from the planet. By varying the planetary gas temperature, two regimes are found. At high temperature, a supersonic planetary wind is found, which is turned around by the stellar wind and forms a tail behind the planet. At lower temperatures, the planetary wind is shut off when the stellar wind penetrates inside where the sonic point would have been. In this regime mass is lost by viscous interaction at the boundary between planetary and stellar wind gases. Absorption by cold hydrogen atoms is large near the planetary surface, and decreases away from the planet as expected. The hot hydrogen absorption is in an annulus and typically dominated by the tail, at large impact parameter, rather than by the thin leading edge of the mixing layer near the substellar point.
PHOTOIONIZATION IN THE SOLAR WIND
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Landi, E.; Lepri, S. T., E-mail: elandi@umich.edu [Department of Climate and Space Sciences and Engineering, University of Michigan, Ann Arbor, MI 48109 (United States)
2015-10-20
In this work we investigate the effects of photoionization on the charge state composition of the solar wind. Using measured solar EUV and X-ray irradiance, the Michigan Ionization Code and a model for the fast and slow solar wind, we calculate the evolution of the charge state distribution of He, C, N, O, Ne, Mg, Si, S, and Fe with and without including photoionization for both types of wind. We find that the solar radiation has significant effects on the charge state distribution of C, N, and O, causing the ionization levels of these elements to be higher than without photoionization; differences are largest for oxygen. The ions commonly observed for elements heavier than O are much less affected, except in ICMEs where Fe ions more ionized than 16+ can also be affected by the solar radiation. We also show that the commonly used O{sup 7+}/O{sup 6+} density ratio is the most sensitive to photoionization; this sensitivity also causes the value of this ratio to depend on the phase of the solar cycle. We show that the O{sup 7+}/O{sup 6+} ratio needs to be used with caution for solar wind classification and coronal temperature estimates, and recommend the C{sup 6+}/C{sup 4+} ratio for these purposes.
International Nuclear Information System (INIS)
Summers, D.
1980-01-01
The theory of stellar winds as given by the equations of classical fluid dynamics is considered. The equations of momentum and energy describing a steady, spherically symmetric, heat-conducting, viscous stellar wind are cast in a dimensionless form which involves a thermal conduction parameter E and a viscosity parameter γ. An asymptotic analysis is carried out, for fixed γ, in the cases E→O and E→infinity (corresponding to small and large thermal conductivity, respectively), and it is found that it is possible to construct critical solutions for the wind velocity and temperature over the entire flow. The E→O solution represents a wind which emanates from the star at low, subsonic speeds, accelerates through a sonic point, and then approaches a constant asymptotic speed, with its temperature varying as r/sup -4/3/ at large distances r from the star; the E→infinity solution represents a wind which, after reaching an approximately constant speed, with temperature varying as r/sup -2/7/, decelerates through a diffuse shock and approaches a finite pressure at infinity. A categorization is made of all critical stellar wind solutions for given values of γ and E, and actual numerical examples are given. Numerical solutions are obtained by integrating upstream 'from infinity' from initial values of the flow parameters given by appropriate asymptotic expansions. The role of viscosity in stellar wind theory is discussed, viscous and inviscid stellar wind solutions are compared, and it is suggested that with certain limitations, the theory presented may be useful in analyzing winds from solar-type stars
Stellar winds in binary X-ray systems
Macgregor, K. B.; Vitello, P. A. J.
1982-01-01
It is thought that accretion from a strong stellar wind by a compact object may be responsible for the X-ray emission from binary systems containing a massive early-type primary. To investigate the effect of X-ray heating and ionization on the mass transfer process in systems of this type, an idealized model is constructed for the flow of a radiation-driven wind in the presence of an X-ray source of specified luminosity, L sub x. It is noted that for low values of L sub x, X-ray photoionization gives rise to additional ions having spectral lines with wavelengths situated near the peak of the primary continuum flux distribution. As a consequence, the radiation force acting on the gas increases in relation to its value in the absence of X-rays, and the wind is accelerated to higher velocities. As L sub x is increased, the degree of ionization of the wind increases, and the magnitude of the radiation force is diminished in comparison with the case in which L sub x = 0. This reduction leads at first to a decrease in the wind velocity and ultimately (for L sub x sufficiently large) to the termination of radiatively driven mass loss.
Astrospheres and Solar-like Stellar Winds
Directory of Open Access Journals (Sweden)
Wood Brian E.
2004-07-01
Full Text Available Stellar analogs for the solar wind have proven to be frustratingly difficult to detect directly. However, these stellar winds can be studied indirectly by observing the interaction regions carved out by the collisions between these winds and the interstellar medium (ISM. These interaction regions are called "astrospheres", analogous to the "heliosphere" surrounding the Sun. The heliosphere and astrospheres contain a population of hydrogen heated by charge exchange processes that can produce enough H I Ly alpha absorption to be detectable in UV spectra of nearby stars from the Hubble Space Telescope (HST. The amount of astrospheric absorption is a diagnostic for the strength of the stellar wind, so these observations have provided the first measurements of solar-like stellar winds. Results from these stellar wind studies and their implications for our understanding of the solar wind are reviewed here. Of particular interest are results concerning the past history of the solar wind and its impact on planetary atmospheres.
Photoionization models for the wind from TW Vir
Kallman, T.
1985-01-01
Line profiles are examined for the resonance doublets of the ions C IV, Si IV, and N V in the spectrum of the dwarf nova TW Virginis as observed by Cordova and Mason (1982). Line strengths depend on the abundances of the scattering ions and hence on the physical characteristics in the stellar wind. Results of the study show that the observed UV line ratios from TW Vir cannot be produced by photoionization by either an unattenuated single bremsstrahlung or by a single blackbody spectrum. Satisfactory values of the abundance ratios can be produced by bremsstrahlung spectra extending into the X-ray region which have low-energy cutoffs near the N IV threshold energy at 77 eV and have fluxes corresponding to an ionization parameter xi-sub-br of about 10. A finding that the flux in the soft X-ray bremsstrahlung component must exceed the EUV blackbody flux by at least an order of magnitude has implications for theories of the continuum emission from cataclysmic variables.
Interacting supernovae from photoionization-confined shells around red supergiant stars
Mackey, Jonathan; Mohamed, Shazrene; Gvaramadze, Vasilii V.; Kotak, Rubina; Langer, Norbert; Meyer, Dominique M.-A.; Moriya, Takashi J.; Neilson, Hilding R.
2014-08-01
Betelgeuse, a nearby red supergiant, is a fast-moving star with a powerful stellar wind that drives a bow shock into its surroundings. This picture has been challenged by the discovery of a dense and almost static shell that is three times closer to the star than the bow shock and has been decelerated by some external force. The two physically distinct structures cannot both be formed by the hydrodynamic interaction of the wind with the interstellar medium. Here we report that a model in which Betelgeuse's wind is photoionized by radiation from external sources can explain the static shell without requiring a new understanding of the bow shock. Pressure from the photoionized wind generates a standing shock in the neutral part of the wind and forms an almost static, photoionization-confined shell. Other red supergiants should have much more massive shells than Betelgeuse, because the photoionization-confined shell traps up to 35 per cent of all mass lost during the red supergiant phase, confining this gas close to the star until it explodes. After the supernova explosion, massive shells dramatically affect the supernova light curve, providing a natural explanation for the many supernovae that have signatures of circumstellar interaction.
Stellar feedback in galaxies and the origin of galaxy-scale winds
Hopkins, Philip F.; Quataert, Eliot; Murray, Norman
2012-04-01
Feedback from massive stars is believed to play a critical role in driving galactic super-winds that enrich the intergalactic medium and shape the galaxy mass function, mass-metallicity relation and other global galaxy properties. In previous papers, we have introduced new numerical methods for implementing stellar feedback on sub-giant molecular cloud (sub-GMC) through galactic scales in numerical simulations of galaxies; the key physical processes include radiation pressure in the ultraviolet through infrared, supernovae (Type I and Type II), stellar winds ('fast' O star through 'slow' asymptotic giant branch winds), and H II photoionization. Here, we show that these feedback mechanisms drive galactic winds with outflow rates as high as ˜10-20 times the galaxy star formation rate. The mass-loading efficiency (wind mass-loss rate divided by the star formation rate) scales roughly as ? (where Vc is the galaxy circular velocity), consistent with simple momentum-conservation expectations. We use our suite of simulations to study the relative contribution of each feedback mechanism to the generation of galactic winds in a range of galaxy models, from Small Magellanic Cloud like dwarfs and Milky Way (MW) analogues to z˜ 2 clumpy discs. In massive, gas-rich systems (local starbursts and high-z galaxies), radiation pressure dominates the wind generation. By contrast, for MW-like spirals and dwarf galaxies the gas densities are much lower and sources of shock-heated gas such as supernovae and stellar winds dominate the production of large-scale outflows. In all of our models, however, the winds have a complex multiphase structure that depends on the interaction between multiple feedback mechanisms operating on different spatial scales and time-scales: any single feedback mechanism fails to reproduce the winds observed. We use our simulations to provide fitting functions to the wind mass loading and velocities as a function of galaxy properties, for use in cosmological
International Nuclear Information System (INIS)
Weymann, R.J.
1978-01-01
It is known that a steady outflow of material at comparable rates of mass loss but vastly different speeds is now known to be ubiquitous phenomenon among both the luminous hot stars and the luminous but cool red giants. The flows are probably massive enough in both cases to give rise to significant effects on stellar evolution and the mass balance between stars and the interstellar medium. The possible mechanisms for these phenomena as well as the methods of observation used are described. In particular, the mass-loss processes in stars other than the sun that also involve a steady flow of matter are considered. The evidence for their existence is described, and then the question of whether the process thought to produce the solar wind is also responsible for producing these stellar winds is explored
Hydrodynamics and stellar winds an introduction
Maciel, Walter J
2014-01-01
Stellar winds are a common phenomenon in the life of stars, from the dwarfs like the Sun to the red giants and hot supergiants, constituting one of the basic aspects of modern astrophysics. Stellar winds are a hydrodynamic phenomenon in which circumstellar gases expand towards the interstellar medium. This book presents an elementary introduction to the fundamentals of hydrodynamics with an application to the study of stellar winds. The principles of hydrodynamics have many other applications, so that the book can be used as an introduction to hydrodynamics for students of physics, astrophysics and other related areas.
The Contribution of Stellar Winds to Cosmic Ray Production
Seo, Jeongbhin; Kang, Hyesung; Ryu, Dongsu
2018-04-01
Massive stars blow powerful stellar winds throughout their evolutionary stages from the main sequence to Wolf-Rayet phases. The wind mechanical energy of a massive star deposited to the interstellar medium can be comparable to the explosion energy of a core-collapse supernova that detonates at the end of its life In this study, we estimate the kinetic energy deposition by massive stars in our Galaxy by considering the integrated Galactic initial mass function and modeling the stellar wind luminosity. The mass loss rate and terminal velocity of stellar winds during the main sequence, red supergiant, and Wolf-Rayet stages are estimated by adopting theoretical calculations and observational data published in the literature. We find that the total stellar wind luminosity by all massive stars in the Galaxy is about Lw ≈ 1.1×1041 ergs, which is about 1/4 of the power of supernova explosions, LSN ≈ 4.8×1041 ergs. If we assume that ˜1-1% of the wind luminosity could be converted to Galactic cosmic rays (GCRs) through collisonless shocks such as termination shocks in stellar bubbles and superbubbles, colliding-wind shocks in binaries, and bow-shocks of massive runaway stars, stellar winds are expected to make a significant contribution to GCR production, though lower than that of supernova remnants.
The Physics of Wind-Fed Accretion
International Nuclear Information System (INIS)
Mauche, Christopher W.; Liedahl, Duane A.; Akiyama, Shizuka; Plewa, Tomasz
2008-01-01
We provide a brief review of the physical processes behind the radiative driving of the winds of OB stars and the Bondi-Hoyle-Lyttleton capture and accretion of a fraction of the stellar wind by a compact object, typically a neutron star, in detached high-mass X-ray binaries (HMXBs). In addition, we describe a program to develop global models of the radiatively-driven photoionized winds and accretion flows of HMXBs, with particular attention to the prototypical system Vela X-l. The models combine XSTAR photoionization calculations, HULLAC emission models appropriate to X-ray photoionized plasmas, improved models of the radiative driving of photoionized winds, FLASH time-dependent adaptive-mesh hydrodynamics calculations, and Monte Carlo radiation transport. We present two- and three-dimensional maps of the density, temperature, velocity, ionization parameter, and emissivity distributions of representative X-ray emission lines, as well as synthetic global Monte Carlo X-ray spectra. Such models help to better constrain the properties of the winds of HMXBs, which bear on such fundamental questions as the long-term evolution of these binaries and the chemical enrichment of the interstellar medium.
Halo Emission of the Cat's Eye Nebula, NGC 6543 Shock Excitation by Fast Stellar Winds
Directory of Open Access Journals (Sweden)
Siek Hyung
2002-09-01
Full Text Available Images taken with the Chandra X-ray telescope have for the the first time revealed the central, wind-driven, hot bubble (Chu et al. 2001, while Hubble Space Telescope (HST WFPC2 images of the Cat's Eye nebula, NGC 6543, show that the temperature of the halo region of angular radius ~ 20'', is much higher than that of the inner bright H II region. With the coupling of a photoionization calculation to a hydrodynamic simulation, we predict the observed [O III] line intensities of the halo region with the same O abundance as in the core H II region: oxygen abundance gradient does not appear to exist in the NGC 6543 inner halo. An interaction between a (leaky fast stellar wind and halo gas may cause the higher excitation temperatures in the halo region and the inner hot bubble region observed with the Chandra X-ray telescope.
Stellar Wind Retention and Expulsion in Massive Star Clusters
Naiman, J. P.; Ramirez-Ruiz, E.; Lin, D. N. C.
2018-05-01
Mass and energy injection throughout the lifetime of a star cluster contributes to the gas reservoir available for subsequent episodes of star formation and the feedback energy budget responsible for ejecting material from the cluster. In addition, mass processed in stellar interiors and ejected as winds has the potential to augment the abundance ratios of currently forming stars, or stars which form at a later time from a retained gas reservoir. Here we present hydrodynamical simulations that explore a wide range of cluster masses, compactnesses, metallicities and stellar population age combinations in order to determine the range of parameter space conducive to stellar wind retention or wind powered gas expulsion in star clusters. We discuss the effects of the stellar wind prescription on retention and expulsion effectiveness, using MESA stellar evolutionary models as a test bed for exploring how the amounts of wind retention/expulsion depend upon the amount of mixing between the winds from stars of different masses and ages. We conclude by summarizing some implications for gas retention and expulsion in a variety of compact (σv ≳ 20 kms-1) star clusters including young massive star clusters (105 ≲ M/M⊙ ≲ 107, age ≲ 500 Myrs), intermediate age clusters (105 ≲ M/M⊙ ≲ 107, age ≈ 1 - 4 Gyrs), and globular clusters (105 ≲ M/M⊙ ≲ 107, age ≳ 10 Gyrs).
Cosmic-ray-modified stellar winds. III. A numerical iterative approach
International Nuclear Information System (INIS)
Ko, C.M.; Jokipii, J.R.; Webb, G.M.
1988-01-01
A numerical iterative method is used to determine the modification of a stellar wind flow with a termination shock by the galactic cosmic rays. A two-fluid model consisting of cosmic rays and thermal stellar wind gas is used in which the cosmic rays are coupled to the background flow via scattering with magnetohydrodynamic waves or irregularities. A polytropic model is used to describe the thermal stellar wind gas, and the cosmic-rays are modeled as a hot, low-density gas with negligible mass flux. The positive galactic cosmic-ray pressure gradient serves to brake the outflowing stellar wind gas, and the cosmic rays modify the location of the critical point of the wind, the location of the shock, the wind fluid velocity profile, and the thermal gas entropy constants on both sides of the shock. The transfer of energy to the cosmic rays results in an outward radial flux of cosmic-ray energy. 21 references
Cosmic-ray acceleration at stellar wind terminal shocks
International Nuclear Information System (INIS)
Webb, G.M.; Forman, M.A.; Axford, W.I.
1985-01-01
Steady-state, spherically symmetric, analytic solutions of the cosmic-ray transport equations, applicable to the problem of acceleration of cosmic rays at the terminal shock to a stellar wind, are studied. The spectra, gradients, and flow patterns of particle modulated and accelerated by the stellar wind and shock are investigated by means of monoenergetic-source solutions at finite radius, as well as solutions with monoenergetic and power-law Galactic spectra. The solutions obtained apply in the test particle limit in which the cosmic rays do not modify the background flow. The solutions show a characteristic power-law momentum spectrum for accelerated particles and a more complex spectrum of particles that are decelerated in the stellar wind. The power-law spectral index depends on the compression ratio of the shock and on the modulation parameters characterizing propagation conditions in the upstream and downstream regions of the shock. Solutions of the transport equations for the total density N (integrated over all energies), pressure P/sub c/, and energy flux F/sub c/ of Galactic cosmic rays interacting with a stellar wind and shock are also studied. The density N(r) increases with radius r, and for strong shocks with large enough modulation parameters, there may be a significant enhancement of the pressure of weakly relativistic particles near the shock compared to the cosmic-ray background pressure P/sub infinity/. The emergent energy flux at infinity is of the order of 4π R 2 V 1 P/sub infinity/ (V 1 is wind velocity upstream of the shock, R is shock radius)
Stellar and wind parameters of massive stars from spectral analysis
Araya, Ignacio; Curé, Michel
2017-11-01
The only way to deduce information from stars is to decode the radiation it emits in an appropriate way. Spectroscopy can solve this and derive many properties of stars. In this work we seek to derive simultaneously the stellar and wind characteristics of a wide range of massive stars. Our stellar properties encompass the effective temperature, the surface gravity, the stellar radius, the micro-turbulence velocity, the rotational velocity and the Si abundance. For wind properties we consider the mass-loss rate, the terminal velocity and the line-force parameters α, k and δ (from the line-driven wind theory). To model the data we use the radiative transport code Fastwind considering the newest hydrodynamical solutions derived with Hydwind code, which needs stellar and line-force parameters to obtain a wind solution. A grid of spectral models of massive stars is created and together with the observed spectra their physical properties are determined through spectral line fittings. These fittings provide an estimation about the line-force parameters, whose theoretical calculations are extremely complex. Furthermore, we expect to confirm that the hydrodynamical solutions obtained with a value of δ slightly larger than ~ 0.25, called δ-slow solutions, describe quite reliable the radiation line-driven winds of A and late B supergiant stars and at the same time explain disagreements between observational data and theoretical models for the Wind-Momentum Luminosity Relationship (WLR).
Stellar winds and molecular clouds: a search for ionized stellar winds
International Nuclear Information System (INIS)
Rodriguez, L.F.; Canto, J.
1983-01-01
We observed with the VLA several regions of mass outflow at 20.6 and 2 cm: LKHα 198, GL 490, HH 7-11, T Tau, GGD 12-15, GL 961, GGD 27-28, V645 CyG, Cep A, and MWC 1080. In most of the regions no continuum source was detected, down to the mJy level, at 6 cm that could be identified as the energy source of the outflow. This result suggests that in these cases the stellar winds powering the outflows are either neutral or, if ionized, have a large terminal velocity (approx. 10 3 km s -1 ). T Tauri and most of the other sources detected show spectra characteristic of an optically-thin H II region and not that of simple ionized winds. We measured the positions of several H 2 O masers associated with mass outflow regions: GL 490, OMC(2)1, Mon R2, GGD 12-15, S106, GL 2591, NGC 7129(2), S140 and Cep A. (author)
National Research Council Canada - National Science Library
Justus, Kristine
2002-01-01
The patterns of stimulus available to moths flying along pheromone plumes in a 3-m-long wind tunnel were characterized using a high frequency photoionization detector in conjunction with an inert tracer gas...
Variable accretion of stellar winds onto Sgr A*
Cuadra, Jorge; Nayakshin, Sergei
2006-12-01
We report a 3-dimensional numerical study of the accretion of stellar winds onto Sgr A*, the super-massive black hole at the centre of our Galaxy. Compared with previous investigations, we allow the stars to be on realistic orbits, include the recently discovered slow wind sources, and allow for optically thin radiative cooling. We frst show the strong inflience of the stellar dynamics on the accretion onto the central black hole. We then present more realistic simulations of Sgr A* accretion and frid that the slow winds shock and rapidly cool, forming cold gas clumps and flaments that coexist with the hot X-ray emitting gas. The accretion rate in this case is highly variable on time-scales of tens to hundreds of years. Such variability can in principle lead to a strongly non-linear response through accretion fbw physics not resolved here, making Sgr A* an important energy source for the Galactic centre.
Variable accretion of stellar winds onto Sgr A*
Energy Technology Data Exchange (ETDEWEB)
Cuadra, Jorge [Max-Planck-Institut fuer Astrophysik, D-85741 Garching (Germany); Nayakshin, Sergei [Department of Physics and Astronomy, University of Leicester, LEI 7RH (United Kingdom)
2006-12-15
We report a 3-dimensional numerical study of the accretion of stellar winds onto Sgr A*, the super-massive black hole at the centre of our Galaxy. Compared with previous investigations, we allow the stars to be on realistic orbits, include the recently discovered slow wind sources, and allow for optically thin radiative cooling. We frst show the strong inflience of the stellar dynamics on the accretion onto the central black hole. We then present more realistic simulations of Sgr A* accretion and frid that the slow winds shock and rapidly cool, forming cold gas clumps and flaments that coexist with the hot X-ray emitting gas. The accretion rate in this case is highly variable on time-scales of tens to hundreds of years. Such variability can in principle lead to a strongly non-linear response through accretion fbw physics not resolved here, making Sgr A* an important energy source for the Galactic centre.
Variable accretion of stellar winds onto Sgr A*
International Nuclear Information System (INIS)
Cuadra, Jorge; Nayakshin, Sergei
2006-01-01
We report a 3-dimensional numerical study of the accretion of stellar winds onto Sgr A*, the super-massive black hole at the centre of our Galaxy. Compared with previous investigations, we allow the stars to be on realistic orbits, include the recently discovered slow wind sources, and allow for optically thin radiative cooling. We frst show the strong inflience of the stellar dynamics on the accretion onto the central black hole. We then present more realistic simulations of Sgr A* accretion and frid that the slow winds shock and rapidly cool, forming cold gas clumps and flaments that coexist with the hot X-ray emitting gas. The accretion rate in this case is highly variable on time-scales of tens to hundreds of years. Such variability can in principle lead to a strongly non-linear response through accretion fbw physics not resolved here, making Sgr A* an important energy source for the Galactic centre
Energy Technology Data Exchange (ETDEWEB)
Wünsch, R.; Palouš, J.; Ehlerová, S. [Astronomical Institute, Academy of Sciences of the Czech Republic, Boční II 1401, 141 31 Prague (Czech Republic); Tenorio-Tagle, G. [Instituto Nacional de Astrofísica Optica y Electrónica, AP 51, 72000 Puebla, México (Mexico)
2017-01-20
We study a model of rapidly cooling shocked stellar winds in young massive clusters and estimate the circumstances under which secondary star formation, out of the reinserted winds from a first stellar generation (1G), is possible. We have used two implementations of the model: a highly idealized, computationally inexpensive, spherically symmetric semi-analytic model, and a complex, three-dimensional radiation-hydrodynamic, simulation; they are in a good mutual agreement. The results confirm our previous findings that, in a cluster with 1G mass 10{sup 7} M {sub ⊙} and half-mass–radius 2.38 pc, the shocked stellar winds become thermally unstable, collapse into dense gaseous structures that partially accumulate inside the cluster, self-shield against ionizing stellar radiation, and form the second generation (2G) of stars. We have used the semi-analytic model to explore a subset of the parameter space covering a wide range of the observationally poorly constrained parameters: the heating efficiency, η {sub he}, and the mass loading, η {sub ml}. The results show that the fraction of the 1G stellar winds accumulating inside the cluster can be larger than 50% if η {sub he} ≲ 10%, which is suggested by the observations. Furthermore, for low η {sub he}, the model provides a self-consistent mechanism predicting 2G stars forming only in the central zones of the cluster. Finally, we have calculated the accumulated warm gas emission in the H30 α recombination line, analyzed its velocity profile, and estimated its intensity for super star clusters in interacting galaxies NGC4038/9 (Antennae) showing that the warm gas should be detectable with ALMA.
Stellar winds and molecular clouds: a search for ionized stellar winds
Energy Technology Data Exchange (ETDEWEB)
Rodriguez, L F; Canto, J
1983-01-01
We observed with the VLA several regions of mass outflow at 20.6 and 2 cm: LKH..cap alpha.. 198, GL 490, HH 7-11, T Tau, GGD 12-15, GL 961, GGD 27-28, V645 CyG, Cep A, and MWC 1080. In most of the regions no continuum source was detected, down to the mJy level, at 6 cm that could be identified as the energy source of the outflow. This result suggests that in these cases the stellar winds powering the outflows are either neutral or, if ionized, have a large terminal velocity (approx. 10/sup 3/ km s/sup -1/). T Tauri and most of the other sources detected show spectra characteristic of an optically-thin H II region and not that of simple ionized winds. We measured the positions of several H/sub 2/O masers associated with mass outflow regions: GL 490, OMC(2)1, Mon R2, GGD 12-15, S106, GL 2591, NGC 7129(2), S140 and Cep A.
The photoionization mechanism of LINERs - Stellar and nonstellar
Ho, Luis C.; Filippenko, Alexei V.
1993-01-01
We present high quality spectroscopic observations of a sample of 14 LINERs. Starlight removal is achieved by the subtraction of a suitable absorption-line 'template' galaxy, allowing accurate measurements of emission lines. We use these line fluxes to examine the possible excitation mechanisms of LINERs. We suggest that LINERs with weak forbidden O I 6300-A emission may be H II regions photoionized by unusually hot O-type stars. LINERs with forbidden O I/H-alpha approximately greater than 1/6 may be powered by photoionization from a nonstellar continuum. This is supported by the detection of broad H-alpha emission, a correlation between line width and critical density, and pointlike X-ray emission in several of these objects.
Cosmic ray-modified stellar winds. I. Solution topologies and singularities
International Nuclear Information System (INIS)
Ko, C.M.; Webb, G.M.
1987-01-01
In the present two-fluid hydrodynamical model for stellar wind flow modification due to its interaction with Galactic cosmic rays, these rays are coupled to the stellar wind by either hydromagnetic wave scattering or background flow irregularity propagation. The background flow is modified by the cosmic rays via their pressure gradient. The system of equations used possesses a line of singularities in (r, u, P/sub c/)-space, or a two-dimensional hypersurface of singularities in (r, u, P/sub c/, dP/sub c/dr)-space, where r, u, and P/sub c/ are respectively the radial distance from the star, the radial wind flow speed, and the cosmic ray pressure. The singular points may be nodes, foci, or saddle points. 64 references
Colliding Stellar Winds Structure and X-ray Emission
Pittard, J. M.; Dawson, B.
2018-04-01
We investigate the structure and X-ray emission from the colliding stellar winds in massive star binaries. We find that the opening angle of the contact discontinuity (CD) is overestimated by several formulae in the literature at very small values of the wind momentum ratio, η. We find also that the shocks in the primary (dominant) and secondary winds flare by ≈20° compared to the CD, and that the entire secondary wind is shocked when η ≲ 0.02. Analytical expressions for the opening angles of the shocks, and the fraction of each wind that is shocked, are provided. We find that the X-ray luminosity Lx∝η, and that the spectrum softens slightly as η decreases.
Gamma rays from active regions in the galaxy: the possible contribution of stellar winds
International Nuclear Information System (INIS)
Cesarsky, C.J.; Montmerle, Thierry.
1982-08-01
Massive stars release a considerable amount of mechanical energy in the form of strong stellar winds. A fraction of this energy may be transferred to relativistic cosmic rays by diffusive shock acceleration at the wind boundary, and/or in the expanding, turbulent wind itself. Massive stars are most frequently found in OB associations, surrounded by H II regions lying at the edge of dense molecular clouds. The interaction of the freshly accelerated particles with matter gives rise to #betta#-ray emission. In this paper, we first briefly review the current knowledge on the energetics of strong stellar winds from O and Wolf-Rayet stars, as well as from T Tauri stars. Taking into account the finite lifetime of these stars, we then proceed to show that stellar winds dominate the energetics of OB associations during the first 4 to 6 million years, after which supernovae take over. In the solar neighborhood, the star formation rate is constant, and a steady-state situation prevails, in which the supernova contribution is found to be dominant. A small, but meaningful fraction of the CO S-B #betta#-ray sources may be fueled by WR and O stellar winds in OB associations, while the power released by T Tauri stars alone is perhaps insufficient to account for the #betta#-ray emission of nearby dark clouds. Finally, we discuss some controversial aspects of the physics of particle acceleration by stellar winds
Cosmic ray acceleration by stellar wind. Simulation for heliosphere
International Nuclear Information System (INIS)
Petukhov, S.I.; Turpanov, A.A.; Nikolaev, V.S.
1985-01-01
The solar wind deceleration by the interstellar medium may result in the existence of the solar wind terminal shock. In this case a certain fraction of thermal particles after being heated at the shock would obtain enough energy to be injected to the regular acceleration process. An analytical solution for the spectrum in the frame of a simplified model that includes particle acceleration at the shock front and adiabatic cooling inside the stellar wind cavity has been derived. It is shown that the acceleration of the solar wind particles at the solar wind terminal shock is capable of providing the total flux, spectrum and radial gradients of the low-energy protons close to one observed in the interplanetary space
The origin of stellar winds: Subatmospheric nonthermal storage modes versus radiation pressure
International Nuclear Information System (INIS)
Cannon, C.J.; Thomas, R.N.
1977-01-01
Most current models of matter-flux in hot stars place its origin in radiation pressure, and then model the flow explicitly to produce no chromosphere-corona. Our model of the stellar atmosphere as a transition zone between stellar interior and interstellar medium places the origin of matter-flux, chromosphere-corona, and spectral ''emission classes'' in subatmospheric nonthermal kinetic energy storage, equally for all stars, hot or cold. Current observations of both hot and cold stars suggest chromospheres to be a universal phenomenon, correlated with matter-fluxes, and enhanced in ''emission-class'' stars. To clarify the difference between the two kinds of models above, we reformulate the wind-tunnel analogy to stellar winds, suggesting that stars satisfy and ''imperfect,'' such model;i.e., transsonic shocks occur before the throat, corresponding to an imposed outward velocity in the storage section, or subatmosphere. We then investigate the stability of an arbitrary stellar atmosphere, hot or cold, to suggest a cause for such an outward subatmospheric velocity
Effects of time-dependent photoionization on interstellar pickup atoms
International Nuclear Information System (INIS)
Isenberg, P.A.; Lee, M.A.
1995-01-01
We present an analytical model for the density variations of interstellar pickup ions in the solar wind due to a time-dependent variation in the photoionization rate, our model predicts a pickup ion density enhancement lasting for a time of the order of the duration of the increase plus the solar wind convection time to the observation point. If the photoionization rate returns to its initial value, this enhancement is followed by a decreased pickup ion density resulting from a depleted interstellar neutral particle density. In the absence of further variations in the photoionization rate, the pickup ion density recovers on a time which scales as the radial position of the observation point divided by the inflow speed of the neutral particles. Gradual variations in the photoionization rate result in a pickup ion density which tends to track the ionization rate, though the density variations are smoothed and delayed in time due to the solar wind convection of ions picked up at points closer to the Sun. 27 refs., 4 figs
Energy Technology Data Exchange (ETDEWEB)
Guzmán, Andrés E.; Garay, Guido; Bronfman, Leonardo; Mardones, Diego [Departamento de Astronomía, Universidad de Chile, Camino el Observatorio 1515, Las Condes, Santiago (Chile); Rodríguez, Luis F. [Centro de Radioastronomía y Astrofísica (UNAM), Morelia 58089 (Mexico); Moran, James [Harvard-Smithsonian Center for Astrophysics, 60 Garden Street, Cambridge, MA (United States); Brooks, Kate J. [CSIRO Astronomy and Space Science, P.O. Box 76, Epping, 1710 NSW (Australia); Nyman, Lars-Åke [Joint ALMA Observatory (JAO), Alonso de Córdova 3107, Vitacura, Santiago (Chile); Sanhueza, Patricio [Institute for Astrophysical Research, Boston University, Boston, MA 02215 (United States)
2014-12-01
We report the detection, made using ALMA, of the 92 GHz continuum and hydrogen recombination lines (HRLs) H40α, H42α, and H50β emission toward the ionized wind associated with the high-mass young stellar object G345.4938+01.4677. This is the luminous central dominating source located in the massive and dense molecular clump associated with IRAS 16562–3959. The HRLs exhibit Voigt profiles, which is a strong signature of Stark broadening. We successfully reproduce the observed continuum and HRLs simultaneously using a simple model of a slow ionized wind in local thermodynamic equilibrium, with no need for a high-velocity component. The Lorentzian line wings imply electron densities of 5 × 10{sup 7} cm{sup –3} on average. In addition, we detect SO and SO{sub 2} emission arising from a compact (∼3000 AU) molecular core associated with the central young star. The molecular core exhibits a velocity gradient that is perpendicular to the jet-axis, which we interpret as evidence of rotation. The set of observations toward G345.4938+01.4677 are consistent with it being a young high-mass star associated with a slow photo-ionized wind.
Two-step photoionization of hydrogen atoms in interplanetary space
International Nuclear Information System (INIS)
Gruntman, M.A.
1990-01-01
Photoionization is one of the key processes which determine the properties of fluxes of neutral atoms in interplanetary space. A new two-step channel (called indirect) of photoionization of hydrogen atoms is proposed. Hydrogen atoms are at first excited to states with principal quantum number n > 2, then decay to metastable H(2S) states, where they can be photoionized. Competing processes due to the interaction with solar wind plasma and solar radiation are considered and the photoionization rate through the proposed indirect channel is calculated. This rate depends on distance from the Sun as ∝ 1/R 4 at large distances (R > 1-2 a.u.) and as ∝ 1/R 2 at close approaches, where it is higher than the rate of direct photoionization. (author)
New method to design stellarator coils without the winding surface
Zhu, Caoxiang; Hudson, Stuart R.; Song, Yuntao; Wan, Yuanxi
2018-01-01
Finding an easy-to-build coils set has been a critical issue for stellarator design for decades. Conventional approaches assume a toroidal ‘winding’ surface, but a poorly chosen winding surface can unnecessarily constrain the coil optimization algorithm, This article presents a new method to design coils for stellarators. Each discrete coil is represented as an arbitrary, closed, one-dimensional curve embedded in three-dimensional space. A target function to be minimized that includes both physical requirements and engineering constraints is constructed. The derivatives of the target function with respect to the parameters describing the coil geometries and currents are calculated analytically. A numerical code, named flexible optimized coils using space curves (FOCUS), has been developed. Applications to a simple stellarator configuration, W7-X and LHD vacuum fields are presented.
Stellar winds and coronae of low-mass Population II/III stars
Suzuki, Takeru K.
2018-06-01
We investigated stellar winds from zero-/low-metallicity low-mass stars by magnetohydrodynamical simulations for stellar winds driven by Alfvén waves from stars with mass M = (0.6-0.8) M⊙ and metallicity Z = (0-1) Z⊙, where M⊙ and Z⊙ are the solar mass and metallicity, respectively. Alfvénic waves, which are excited by the surface convection, travel upward from the photosphere and heat up the corona by their dissipation. For lower Z, denser gas can be heated up to the coronal temperature because of the inefficient radiation cooling. The coronal density of Population II/III stars with Z ≤ 0.01 Z⊙ is one to two orders of magnitude larger than that of a solar-metallicity star with the same mass, and as a result, the mass loss rate, \\dot{M}, is 4.5-20 times larger. This indicates that metal accretion on low-mass Pop. III stars is negligible. The soft X-ray flux of the Pop. II/III stars is also expected to be ˜1-30 times larger than that of a solar-metallicity counterpart owing to the larger coronal density, even though the radiation cooling efficiency is smaller. A larger fraction of the input Alfvénic wave energy is transmitted to the corona in low-Z stars because they avoid severe reflection owing to the smaller density difference between the photosphere and the corona. Therefore, a larger fraction is converted to the thermal energy of the corona and the kinetic energy of the stellar wind. From this energetics argument, we finally derived a scaling of \\dot{M} as \\dot{M}∝ L R_{\\star }^{11/9} M_{\\star }^{-10/9} T_eff^{11/2}[\\max (Z/Z_{⊙},0.01)]^{-1/5}, where L, R⋆, and Teff are the stellar luminosity, radius, and effective temperature, respectively.
Stellar winds and coronae of low-mass Population II/III stars
Suzuki, Takeru K.
2018-04-01
We investigated stellar winds from zero-/low-metallicity low-mass stars by magnetohydrodynamical simulations for stellar winds driven by Alfvén waves from stars with mass M = (0.6-0.8) M⊙ and metallicity Z = (0-1) Z⊙, where M⊙ and Z⊙ are the solar mass and metallicity, respectively. Alfvénic waves, which are excited by the surface convection, travel upward from the photosphere and heat up the corona by their dissipation. For lower Z, denser gas can be heated up to the coronal temperature because of the inefficient radiation cooling. The coronal density of Population II/III stars with Z ≤ 0.01 Z⊙ is one to two orders of magnitude larger than that of a solar-metallicity star with the same mass, and as a result, the mass loss rate, \\dot{M}, is 4.5-20 times larger. This indicates that metal accretion on low-mass Pop. III stars is negligible. The soft X-ray flux of the Pop. II/III stars is also expected to be ˜1-30 times larger than that of a solar-metallicity counterpart owing to the larger coronal density, even though the radiation cooling efficiency is smaller. A larger fraction of the input Alfvénic wave energy is transmitted to the corona in low-Z stars because they avoid severe reflection owing to the smaller density difference between the photosphere and the corona. Therefore, a larger fraction is converted to the thermal energy of the corona and the kinetic energy of the stellar wind. From this energetics argument, we finally derived a scaling of \\dot{M} as \\dot{M}∝ L R_{\\star }^{11/9} M_{\\star }^{-10/9} T_eff^{11/2}[\\max (Z/Z_{⊙},0.01)]^{-1/5}, where L, R⋆, and Teff are the stellar luminosity, radius, and effective temperature, respectively.
Wind bubbles within H ii regions around slowly moving stars
Mackey, Jonathan; Gvaramadze, Vasilii V.; Mohamed, Shazrene; Langer, Norbert
2015-01-01
Interstellar bubbles around O stars are driven by a combination of the star's wind and ionizing radiation output. The wind contribution is uncertain because the boundary between the wind and interstellar medium is difficult to observe. Mid-infrared observations (e.g., of the H ii region RCW 120) show arcs of dust emission around O stars, contained well within the H ii region bubble. These arcs could indicate the edge of an asymmetric stellar wind bubble, distorted by density gradients and/or stellar motion. We present two-dimensional, radiation-hydrodynamics simulations investigating the evolution of wind bubbles and H ii regions around massive stars moving through a dense (nH = 3000 cm-3), uniform medium with velocities ranging from 4 to 16 km s-1. The H ii region morphology is strongly affected by stellar motion, as expected, but the wind bubble is also very aspherical from birth, even for the lowest space velocity considered. Wind bubbles do not fill their H ii regions (we find filling factors of 10-20 per cent), at least for a main sequence star with mass M⋆ ~ 30 M⊙. Furthermore, even for supersonic velocities the wind bow shock does not significantly trap the ionization front. X-ray emission from the wind bubble is soft, faint, and comes mainly from the turbulent mixing layer between the wind bubble and the H ii region. The wind bubble radiates <1 per cent of its energy in X-rays; it loses most of its energy by turbulent mixing with cooler photoionized gas. Comparison of the simulations with the H ii region RCW 120 shows that its dynamical age is ≲0.4 Myr and that stellar motion ≲4 km s-1 is allowed, implying that the ionizing source is unlikely to be a runaway star but more likely formed in situ. The region's youth, and apparent isolation from other O or B stars, makes it very interesting for studies of massive star formation and of initial mass functions. Movies are available in electronic form at http://www.aanda.org
THERMAL X-RAY EMISSION FROM THE SHOCKED STELLAR WIND OF PULSAR GAMMA-RAY BINARIES
Energy Technology Data Exchange (ETDEWEB)
Zabalza, V.; Paredes, J. M. [Departament d' Astronomia i Meteorologia, Institut de Ciencies del Cosmos (ICC), Universitat de Barcelona (IEEC-UB), Marti i Franques 1, E08028 Barcelona (Spain); Bosch-Ramon, V., E-mail: vzabalza@am.ub.es [Dublin Institute for Advanced Studies, 31 Fitzwilliam Place, Dublin 2 (Ireland)
2011-12-10
Gamma-ray-loud X-ray binaries are binary systems that show non-thermal broadband emission from radio to gamma rays. If the system comprises a massive star and a young non-accreting pulsar, their winds will collide producing broadband non-thermal emission, most likely originated in the shocked pulsar wind. Thermal X-ray emission is expected from the shocked stellar wind, but until now it has neither been detected nor studied in the context of gamma-ray binaries. We present a semi-analytic model of the thermal X-ray emission from the shocked stellar wind in pulsar gamma-ray binaries, and find that the thermal X-ray emission increases monotonically with the pulsar spin-down luminosity, reaching luminosities of the order of 10{sup 33} erg s{sup -1}. The lack of thermal features in the X-ray spectrum of gamma-ray binaries can then be used to constrain the properties of the pulsar and stellar winds. By fitting the observed X-ray spectra of gamma-ray binaries with a source model composed of an absorbed non-thermal power law and the computed thermal X-ray emission, we are able to derive upper limits on the spin-down luminosity of the putative pulsar. We applied this method to LS 5039, the only gamma-ray binary with a radial, powerful wind, and obtain an upper limit on the pulsar spin-down luminosity of {approx}6 Multiplication-Sign 10{sup 36} erg s{sup -1}. Given the energetic constraints from its high-energy gamma-ray emission, a non-thermal to spin-down luminosity ratio very close to unity may be required.
A new mechanical stellar wind feedback model for the Rosette Nebula
Wareing, C. J.; Pittard, J. M.; Wright, N. J.; Falle, S. A. E. G.
2018-04-01
The famous Rosette Nebula has an evacuated central cavity formed from the stellar winds ejected from the 2-6 Myr old codistant and comoving central star cluster NGC 2244. However, with upper age estimates of less than 110 000 yr, the central cavity is too young compared to NGC 2244 and existing models do not reproduce its properties. A new proper motion study herein using Gaia data reveals the ejection of the most massive star in the Rosette, HD 46223, from NGC 2244 occurred 1.73 (+0.34, -0.25) Myr (1σ uncertainty) in the past. Assuming this ejection was at the birth of the most massive stars in NGC 2244, including the dominant centrally positioned HD 46150, the age is set for the famous ionized region at more than 10 times that derived for the cavity. Here, we are able to reproduce the structure of the Rosette Nebula, through simulation of mechanical stellar feedback from a 40 M⊙ star in a thin sheet-like molecular cloud. We form the 135 000 M⊙ cloud from thermally unstable diffuse interstellar medium (ISM) under the influence of a realistic background magnetic field with thermal/magnetic pressure equilibrium. Properties derived from a snapshot of the simulation at 1.5 Myr, including cavity size, stellar age, magnetic field, and resulting inclination to the line of sight, match those derived from observations. An elegant explanation is thus provided for the stark contrast in age estimates based on realistic diffuse ISM properties, molecular cloud formation and stellar wind feedback.
SPIN EVOLUTION OF ACCRETING YOUNG STARS. II. EFFECT OF ACCRETION-POWERED STELLAR WINDS
International Nuclear Information System (INIS)
Matt, Sean P.; Pinzón, Giovanni; Greene, Thomas P.; Pudritz, Ralph E.
2012-01-01
We present a model for the rotational evolution of a young, solar-mass star interacting magnetically with an accretion disk. As in a previous paper (Paper I), the model includes changes in the star's mass and radius as it descends the Hayashi track, a decreasing accretion rate, and a prescription for the angular momentum transfer between the star and disk. Paper I concluded that, for the relatively strong magnetic coupling expected in real systems, additional processes are necessary to explain the existence of slowly rotating pre-main-sequence stars. In the present paper, we extend the stellar spin model to include the effect of a spin-down torque that arises from an accretion-powered stellar wind (APSW). For a range of magnetic field strengths, accretion rates, initial spin rates, and mass outflow rates, the modeled stars exhibit rotation periods within the range of 1-10 days in the age range of 1-3 Myr. This range coincides with the bulk of the observed rotation periods, with the slow rotators corresponding to stars with the lowest accretion rates, strongest magnetic fields, and/or highest stellar wind mass outflow rates. We also make a direct, quantitative comparison between the APSW scenario and the two types of disk-locking models (namely, the X-wind and Ghosh and Lamb type models) and identify some remaining theoretical issues for understanding young star spins.
Detecting stellar-wind bubbles through infrared arcs in H II regions
Mackey, Jonathan; Haworth, Thomas J.; Gvaramadze, Vasilii V.; Mohamed, Shazrene; Langer, Norbert; Harries, Tim J.
2016-02-01
Mid-infrared arcs of dust emission are often seen near ionizing stars within H II regions. A possible explanations for these arcs is that they could show the outer edges of asymmetric stellar wind bubbles. We use two-dimensional, radiation-hydrodynamics simulations of wind bubbles within H II regions around individual stars to predict the infrared emission properties of the dust within the H II region. We assume that dust and gas are dynamically well-coupled and that dust properties (composition, size distribution) are the same in the H II region as outside it, and that the wind bubble contains no dust. We post-process the simulations to make synthetic intensity maps at infrared wavebands using the torus code. We find that the outer edge of a wind bubble emits brightly at 24 μm through starlight absorbed by dust grains and re-radiated thermally in the infrared. This produces a bright arc of emission for slowly moving stars that have asymmetric wind bubbles, even for cases where there is no bow shock or any corresponding feature in tracers of gas emission. The 24 μm intensity decreases exponentially from the arc with increasing distance from the star because the dust temperature decreases with distance. The size distribution and composition of the dust grains has quantitative but not qualitative effects on our results. Despite the simplifications of our model, we find good qualitative agreement with observations of the H II region RCW 120, and can provide physical explanations for any quantitative differences. Our model produces an infrared arc with the same shape and size as the arc around CD -38°11636 in RCW 120, and with comparable brightness. This suggests that infrared arcs around O stars in H II regions may be revealing the extent of stellar wind bubbles, although we have not excluded other explanations.
Gemini/GNIRS infrared spectroscopy of the Wolf-Rayet stellar wind in Cygnus X-3
Koljonen, K. I. I.; Maccarone, T. J.
2017-12-01
The microquasar Cygnus X-3 was observed several times with the Gemini North Infrared Spectrograph while the source was in the hard X-ray state. We describe the observed 1.0-2.4 μm spectra as arising from the stellar wind of the companion star and suggest its classification as a WN 4-6 Wolf-Rayet star. We attribute the orbital variations of the emission line profiles to the variations in the ionization structure of the stellar wind caused by the intense X-ray emission from the compact object. The strong variability observed in the line profiles will affect the mass function determination. We are unable to reproduce earlier results, from which the mass function for the Wolf-Rayet star was derived. Instead, we suggest that the system parameters are difficult to obtain from the infrared spectra. We find that the near-infrared continuum and the line spectra can be represented with non-LTE Wolf-Rayet atmosphere models if taking into account the effects arising from the peculiar ionization structure of the stellar wind in an approximative manner. From the representative models we infer the properties of the Wolf-Rayet star and discuss possible mass ranges for the binary components.
Harbach, Laura Marshall; Drake, Jeremy J.; Garraffo, Cecilia; Alvarado-Gomez, Julian D.; Moschou, Sofia P.; Cohen, Ofer
2018-01-01
Recently, three rocky planets were discovered in the habitable zone of the nearby planetary system TRAPPIST-1. The increasing number of exoplanet detections has led to further research into the planetary requirements for sustaining life. Habitable zone occupants have, in principle, the capacity to retain liquid water, whereas actual habitability might depend on atmospheric retention. However, stellar winds and photon radiation interactions with the planet can lead to severe atmospheric depletion and have a catastrophic impact on a planet’s habitability. While the implications of photoevaporation on atmospheric erosion have been researched to some degree, the influence of stellar winds and Coronal Mass Ejections (CMEs) has yet to be analyzed in detail. Here, we model the effect of the stellar wind and CMEs on the atmospheric envelope of a planet situated in the orbit of TRAPPIST-1e using 3D magnetohydrodynamic (MHD) simulations. In particular, we discuss the atmospheric loss due to the effect of a CME, and the relevance of the stellar and planetary magnetic fields on the sustainability of M-dwarf exoplanetary atmospheres.
The design construction and installation of the helical winding for the CLEO stellarator
International Nuclear Information System (INIS)
Hunt, R.R.; Bayes, D.V.
1979-03-01
The CLEO stellarator has a torus 900mm major radius and 166mm minor radius, fitted externally with a 7 field period, l = 3, 120kAT helical winding of 179mm mean radius. The winding and torus have to withstand the large forces produced by the interaction of the current flowing in the winding with the toroidal magnetic field of 2 tesla produced by 24 coils spaced around the torus. To allow the torus to be divided the winding has to be split requiring a total of 240 demountable current-carrying joints at the torus vacuum joint positions. The design, development, manufacture, installation and operation of the helical winding is discussed. From the early development stages to installation took four years. When completed this was the largest installation of its type in Europe. (author)
DEVIATION OF STELLAR ORBITS FROM TEST PARTICLE TRAJECTORIES AROUND SGr A* DUE TO TIDES AND WINDS
International Nuclear Information System (INIS)
Psaltis, Dimitrios; Li, Gongjie; Loeb, Abraham
2013-01-01
Monitoring the orbits of stars around Sgr A* offers the possibility of detecting the precession of their orbital planes due to frame dragging, of measuring the spin and quadrupole moment of the black hole, and of testing the no-hair theorem. Here we investigate whether the deviations of stellar orbits from test-particle trajectories due to wind mass loss and tidal dissipation of the orbital energy compromise such measurements. We find that the effects of stellar winds are, in general, negligible. On the other hand, for the most eccentric orbits (e > 0.96) for which an optical interferometer, such as GRAVITY, will detect orbital plane precession due to frame dragging, the tidal dissipation of orbital energy occurs at timescales comparable to the timescale of precession due to the quadrupole moment of the black hole. As a result, this non-conservative effect is a potential source of systematic uncertainty in testing the no-hair theorem with stellar orbits
DEVIATION OF STELLAR ORBITS FROM TEST PARTICLE TRAJECTORIES AROUND SGr A* DUE TO TIDES AND WINDS
Energy Technology Data Exchange (ETDEWEB)
Psaltis, Dimitrios [Astronomy Department, University of Arizona, 933 North Cherry Avenue, Tucson, AZ 85721 (United States); Li, Gongjie; Loeb, Abraham, E-mail: dpsaltis@email.arizona.edu, E-mail: gli@cfa.harvard.edu, E-mail: aloeb@cfa.harvard.edu [Institute for Theory and Computation, Harvard-Smithsonian CfA, 60 Garden Street, Cambridge, MA (United States)
2013-11-01
Monitoring the orbits of stars around Sgr A* offers the possibility of detecting the precession of their orbital planes due to frame dragging, of measuring the spin and quadrupole moment of the black hole, and of testing the no-hair theorem. Here we investigate whether the deviations of stellar orbits from test-particle trajectories due to wind mass loss and tidal dissipation of the orbital energy compromise such measurements. We find that the effects of stellar winds are, in general, negligible. On the other hand, for the most eccentric orbits (e > 0.96) for which an optical interferometer, such as GRAVITY, will detect orbital plane precession due to frame dragging, the tidal dissipation of orbital energy occurs at timescales comparable to the timescale of precession due to the quadrupole moment of the black hole. As a result, this non-conservative effect is a potential source of systematic uncertainty in testing the no-hair theorem with stellar orbits.
X-ray emission due to interaction of SN1987A ejecta with its progenitor's stellar-wind matter
International Nuclear Information System (INIS)
Masai, Kuniaki.
1990-06-01
The progenitor of the supernova 1987A, Sk-69 202 probably had lost a considerable amount of mass in its stellar wind in the past evolutionary track through a red supergiant to a blue supergiant. In about 10 years, the expanding ejecta of SN1987A will catch up to collide with the wind matter ejected in the red supergiant phase. Shocks due to the collision will heat up the ejecta and the wind matter to cause an enhancement of thermal X-ray emission lasting for several decades. We predict the X-ray light curve and the spectrum as well as the epoch of the enhancement intending to encourage future X-ray observations, which will give a clue for the study of such peculiar stellar evolution with a blueward transition as Sk-69 202. (author)
Optimization of a stellarator design including modulation of the helical winding geometry
International Nuclear Information System (INIS)
Sharp, L.E.; Petersen, L.F.; Blamey, J.W.
1979-06-01
The optimization of the helical winding geometry of the next generation of high performance stellarators is of critical importance as the current in the helical conductors must be kept to a minimum to reduce the very large electromechanical forces on the conductors. Using a modified version of the Culham computer code MAGBAT, steps towards optimization are described
Photoionization modeling of the LWS fine-structure lines in IR bright galaxies
Satyapal, S.; Luhman, M. L.; Fischer, J.; Greenhouse, M. A.; Wolfire, M. G.
1997-01-01
The long wavelength spectrometer (LWS) fine structure line spectra from infrared luminous galaxies were modeled using stellar evolutionary synthesis models combined with photoionization and photodissociation region models. The calculations were carried out by using the computational code CLOUDY. Starburst and active galactic nuclei models are presented. The effects of dust in the ionized region are examined.
Nebular Continuum and Line Emission in Stellar Population Synthesis Models
Energy Technology Data Exchange (ETDEWEB)
Byler, Nell; Dalcanton, Julianne J. [Department of Astronomy, University of Washington, Box 351580, Seattle, WA 98195 (United States); Conroy, Charlie; Johnson, Benjamin D., E-mail: ebyler@astro.washington.edu [Department of Astronomy, Harvard University, Cambridge, MA 02138 (United States)
2017-05-01
Accounting for nebular emission when modeling galaxy spectral energy distributions (SEDs) is important, as both line and continuum emissions can contribute significantly to the total observed flux. In this work, we present a new nebular emission model integrated within the Flexible Stellar Population Synthesis code that computes the line and continuum emission for complex stellar populations using the photoionization code Cloudy. The self-consistent coupling of the nebular emission to the matched ionizing spectrum produces emission line intensities that correctly scale with the stellar population as a function of age and metallicity. This more complete model of galaxy SEDs will improve estimates of global gas properties derived with diagnostic diagrams, star formation rates based on H α , and physical properties derived from broadband photometry. Our models agree well with results from other photoionization models and are able to reproduce observed emission from H ii regions and star-forming galaxies. Our models show improved agreement with the observed H ii regions in the Ne iii/O ii plane and show satisfactory agreement with He ii emission from z = 2 galaxies, when including rotating stellar models. Models including post-asymptotic giant branch stars are able to reproduce line ratios consistent with low-ionization emission regions. The models are integrated into current versions of FSPS and include self-consistent nebular emission predictions for MIST and Padova+Geneva evolutionary tracks.
Instabilities of line-driven stellar winds. V. Effect of an optically thick continuum
International Nuclear Information System (INIS)
Owocki, S.P.; Rybicki, G.B.
1991-01-01
Earlier analyses of the linear instability of line-driven stellar winds are extended to the case, relevant to Wolf-Rayet stars, in which the continuum remains optically thick well above the sonic point. It is found that an optically thick flow driven by pure scattering lines is stabilized by the drag effect of the diffuse, scattered radiation. However, even a relatively small photon destruction probability can cause a flow with continuum optical thickness much greater than 1 to remain unstable, with a given growth rate. The implications of these results for the variability characteristics of winds from Wolf-Rayet stars are briefly discussed. 16 refs
Recent advances in non-LTE stellar atmosphere models
Sander, Andreas A. C.
2017-11-01
In the last decades, stellar atmosphere models have become a key tool in understanding massive stars. Applied for spectroscopic analysis, these models provide quantitative information on stellar wind properties as well as fundamental stellar parameters. The intricate non-LTE conditions in stellar winds dictate the development of adequate sophisticated model atmosphere codes. The increase in both, the computational power and our understanding of physical processes in stellar atmospheres, led to an increasing complexity in the models. As a result, codes emerged that can tackle a wide range of stellar and wind parameters. After a brief address of the fundamentals of stellar atmosphere modeling, the current stage of clumped and line-blanketed model atmospheres will be discussed. Finally, the path for the next generation of stellar atmosphere models will be outlined. Apart from discussing multi-dimensional approaches, I will emphasize on the coupling of hydrodynamics with a sophisticated treatment of the radiative transfer. This next generation of models will be able to predict wind parameters from first principles, which could open new doors for our understanding of the various facets of massive star physics, evolution, and death.
International Nuclear Information System (INIS)
Moroz, P.E.
1997-03-01
A novel concept for magnetic plasma confinement, Stellarator-Spheromak (SSP), is proposed. Numerical analysis with the classical-stellarator-type outboard stellarator windings demonstrates a number of potential advantages of SSP for controlled nuclear fusion. Among the main ones are: simple and compact magnet coil configuration, absence of material structures (e.g. magnet coils or conducting walls) in the center of the torus, high rotational transform, and a possibility of MHD equilibria with very high β (pressure/magnetic pressure) of the confined plasma
Hydrodynamic Simulations of the Inner Accretion Flow of Sagittarius A* Fueled By Stellar Winds
Ressler, S. M.; Quataert, E.; Stone, J. M.
2018-05-01
We present Athena++ grid-based, hydrodynamic simulations of accretion onto Sagittarius A* via the stellar winds of the ˜30 Wolf-Rayet stars within the central parsec of the galactic center. These simulations span ˜ 4 orders of magnitude in radius, reaching all the way down to 300 gravitational radii of the black hole, ˜32 times further in than in previous work. We reproduce reasonably well the diffuse thermal X-ray emission observed by Chandra in the central parsec. The resulting accretion flow at small radii is a superposition of two components: 1) a moderately unbound, sub-Keplerian, thick, pressure-supported disc that is at most (but not all) times aligned with the clockwise stellar disc, and 2) a bound, low-angular momentum inflow that proceeds primarily along the southern pole of the disc. We interpret this structure as a natural consequence of a few of the innermost stellar winds dominating accretion, which produces a flow with a broad distribution of angular momentum. Including the star S2 in the simulation has a negligible effect on the flow structure. Extrapolating our results from simulations with different inner radii, we find an accretion rate of ˜ a few × 10-8M⊙/yr at the horizon scale, consistent with constraints based on modeling the observed emission of Sgr A*. The flow structure found here can be used as more realistic initial conditions for horizon scale simulations of Sgr A*.
Gadolinium photoionization process
Paisner, Jeffrey A.; Comaskey, Brian J.; Haynam, Christopher A.; Eggert, Jon H.
1993-01-01
A method is provided for selective photoionization of the odd-numbered atomic mass gadolinium isotopes 155 and 157. The selective photoionization is accomplished by circular or linear parallel polarized laser beam energy effecting a three-step photoionization pathway.
STAR CLUSTER FORMATION WITH STELLAR FEEDBACK AND LARGE-SCALE INFLOW
International Nuclear Information System (INIS)
Matzner, Christopher D.; Jumper, Peter H.
2015-01-01
During star cluster formation, ongoing mass accretion is resisted by stellar feedback in the form of protostellar outflows from the low-mass stars and photo-ionization and radiation pressure feedback from the massive stars. We model the evolution of cluster-forming regions during a phase in which both accretion and feedback are present and use these models to investigate how star cluster formation might terminate. Protostellar outflows are the strongest form of feedback in low-mass regions, but these cannot stop cluster formation if matter continues to flow in. In more massive clusters, radiation pressure and photo-ionization rapidly clear the cluster-forming gas when its column density is too small. We assess the rates of dynamical mass ejection and of evaporation, while accounting for the important effect of dust opacity on photo-ionization. Our models are consistent with the census of protostellar outflows in NGC 1333 and Serpens South and with the dust temperatures observed in regions of massive star formation. Comparing observations of massive cluster-forming regions against our model parameter space, and against our expectations for accretion-driven evolution, we infer that massive-star feedback is a likely cause of gas disruption in regions with velocity dispersions less than a few kilometers per second, but that more massive and more turbulent regions are too strongly bound for stellar feedback to be disruptive
Martínez-Núñez, Silvia; Kretschmar, Peter; Bozzo, Enrico; Oskinova, Lidia M.; Puls, Joachim; Sidoli, Lara; Sundqvist, Jon Olof; Blay, Pere; Falanga, Maurizio; Fürst, Felix; Gímenez-García, Angel; Kreykenbohm, Ingo; Kühnel, Matthias; Sander, Andreas; Torrejón, José Miguel; Wilms, Jörn
2017-10-01
Massive stars, at least ˜10 times more massive than the Sun, have two key properties that make them the main drivers of evolution of star clusters, galaxies, and the Universe as a whole. On the one hand, the outer layers of massive stars are so hot that they produce most of the ionizing ultraviolet radiation of galaxies; in fact, the first massive stars helped to re-ionize the Universe after its Dark Ages. Another important property of massive stars are the strong stellar winds and outflows they produce. This mass loss, and finally the explosion of a massive star as a supernova or a gamma-ray burst, provide a significant input of mechanical and radiative energy into the interstellar space. These two properties together make massive stars one of the most important cosmic engines: they trigger the star formation and enrich the interstellar medium with heavy elements, that ultimately leads to formation of Earth-like rocky planets and the development of complex life. The study of massive star winds is thus a truly multidisciplinary field and has a wide impact on different areas of astronomy. In recent years observational and theoretical evidences have been growing that these winds are not smooth and homogeneous as previously assumed, but rather populated by dense "clumps". The presence of these structures dramatically affects the mass loss rates derived from the study of stellar winds. Clump properties in isolated stars are nowadays inferred mostly through indirect methods (i.e., spectroscopic observations of line profiles in various wavelength regimes, and their analysis based on tailored, inhomogeneous wind models). The limited characterization of the clump physical properties (mass, size) obtained so far have led to large uncertainties in the mass loss rates from massive stars. Such uncertainties limit our understanding of the role of massive star winds in galactic and cosmic evolution. Supergiant high mass X-ray binaries (SgXBs) are among the brightest X
Photoionization of excited atoms and ions: recent progress and future prospects
International Nuclear Information System (INIS)
Wuilleumier, F.J.
2004-01-01
Full text: Photoionization of atoms in the ground state using synchrotron radiation (SR) has contributed extensively to a better knowledge of atomic structure and of its dynamical response to photon interaction. Since the st use in 1963 of an SR facility in the ultraviolet to investigate autoionizing states in helium, each improvement in the performance of available SR beams has allowed to go deeper and deeper into the understanding of isolated atomic systems. The study of very dilute targets such as atoms prepared in selected excited states or multiply-charged ions is more challenging. Using dye lasers, the excited state can be prepared with a well defined set of quantum numbers and SR photoionization of this prepared state can be studied as a function of photon energy and emission-angle. For ions, the equivalent ionic densities achievable in a merged-beam experiment do not exceed, usually, 10 6 cm -3 , i.e. they are lower by 5 orders of magnitude than for atoms in the ground state. This explains why the response of ionized matter to photoionizing radiation has been largely unexplored until recently. Theoretical methods, still to be tested by experimental measurements, have been developed to model stellar atmospheres as well as laboratory plasmas. After the pioneering experiments using plasma discharge technology and laser-produced plasmas to measure photoionization in excited states and ions, the use of SR has allowed to dramatically improve experiments for excited- and ionic-species, starting with the first measurements of electron spectra from photoionization of laser-excited sodium atoms, and with the first determination of doubly-charged ion rate resulting from photoionization of singly-charged ions in merged beam experiments. Over the past 5 years, photoionization of singly- and multiply-charged ions using the merged beam technique has been intensively performed at four SR facilities (ASTRID, Spring-8, the Advanced Light Source (ALS), and Super-ACO), all of
Closed and open magnetic fields in stellar winds
Mullan, D. J.; Steinolfson, R. S.
1983-01-01
A numerical study of the interaction between a thermal wind and a global dipole field in the sun and in a giant star is reported. In order for closed field lines to persist near the equator (where a helmet-streamer-like configuration appears), the coronal temperature must be less than a critical value Tc, which scales as M/R. This condition is found to be equivalent to the following: for a static helmet streamer to persist, the sonic point above the helmet must not approach closer to the star than 2.2-2.6 stellar radii. Implications for rapid mass loss and X-ray emission from cool giants are pointed out. The results strengthen the case for identifying empirical dividing lines in the H-R diagram with a magnetic topology transition locus (MTTL). Support for the MTTL concept is also provided by considerations of the breakdown of magnetostatic equilibrium.
International Nuclear Information System (INIS)
Souza Pellegrini, P.S. de.
1976-08-01
The charge exchange reactions: C +2 + H sub(e) 0 → H +1 + C +1 and C +2 + H 0 → H +1 + C +1 were taken into account in the ionization equilibrium of Carbon in photoionization models for line emitting regions of quasi-stellar objects. The new ionization structure of Carbon was obtained and the intensities of the most important emission lines of this element usually observed in QSO's with large redshifts were calculated. The charge exchange with Hidrogen produces negligible effects while the importance of taking into account the charge exchange with Helium can be seen from the change of the ionization structure of Carbon in all considered models. The homogeneous optically thin model is shown not to be consistent with the observations. For non homogeneous optically thick models observable changes in line intensities occur when in the region where charge exhange is dominant the electron density is high enough to produce collisional excitation and consequent line emission. (Author)
Assisted stellar suicide: the wind-driven evolution of the recurrent nova T Pyxidis
Knigge, Ch.; King, A. R.; Patterson, J.
2000-12-01
We show that the extremely high luminosity of the short-period recurrent nova T Pyx in quiescence can be understood if this system is a wind-driven supersoft x-ray source (SSS). In this scenario, a strong, radiation-induced wind is excited from the secondary star and accelerates the binary evolution. The accretion rate is therefore much higher than in an ordinary cataclysmic binary at the same orbital period, as is the luminosity of the white dwarf primary. In the steady state, the enhanced luminosity is just sufficient to maintain the wind from the secondary. The accretion rate and luminosity predicted by the wind-driven model for T Pyx are in good agreement with the observational evidence. X-ray observations with Chandra or XMM may be able to confirm T Pyx's status as a SSS. T Pyx's lifetime in the wind-driven state is on the order of a million years. Its ultimate fate is not certain, but the system may very well end up destroying itself, either via the complete evaporation of the secondary star, or in a Type Ia supernova if the white dwarf reaches the Chandrasekhar limit. Thus either the primary, the secondary, or both may currently be committing assisted stellar suicide.
Density-matrix formalism for the photoion-electron entanglement in atomic photoionization
International Nuclear Information System (INIS)
Radtke, T.; Fritzsche, S.; Surzhykov, A.
2006-01-01
The density-matrix theory, based on Dirac's relativistic equation, is applied for studying the entanglement between the photoelectron and residual ion in the course of the photoionization of atoms and ions. In particular, emphasis is placed on deriving the final-state density matrix of the overall system 'photoion+electron', including interelectronic effects and the higher multipoles of the radiation field. This final-state density matrix enables one immediately to analyze the change of entanglement as a function of the energy, angle and the polarization of the incoming light. Detailed computations have been carried out for the 5s photoionization of neutral strontium, leading to a photoion in a 5s 2 S J f =1/2 level. It is found that the photoion-electron entanglement decreases significantly near the ionization threshold and that, in general, it depends on both the photon energy and angle. The possibility to extract photoion-electron pairs with a well-defined degree of entanglement may have far-reaching consequences for quantum information and elsewhere
International Nuclear Information System (INIS)
Olson, G.L.
1979-01-01
Several models for the winds of O stars have been proposed to explain the unexpected presence of high ionization potential ions such as N +4 and O +5 . Lamers and Snow (1978) proposed that the winds of stars showing N V and O VI lines have elevated temperatures near 4 +- 2 x 10 5 K while cooler stars with anomalous Si IV lines have Tsub(e) approximately 7+-3 x 10 4 K. Alternately, Cassinelli and Olson (1978, CO) and Olson (1978) have explained the presence of these ions by showing that a thin corona at the base of a cool wind (Tsub(e) < approximately Tsub(eff)) can produce these ions by the Auger photoionization process where a single X-ray photon causes the ejection of two electrons. A third possibility is that the winds are at only slightly elevated temperatures (40 000 to 60 000K) and photoionization in an optically thick wind produces the unexpected ions. The present analysis tests the ability of these three wind models to fit the observations of zeta Orionis A 09.7 Ib. (Auth.)
Energy Technology Data Exchange (ETDEWEB)
Cohen, O. [Lowell Center for Space Science and Technology, University of Massachusetts, Lowell, MA 01854 (United States)
2017-02-01
The development of the Zeeman–Doppler Imaging (ZDI) technique has provided synoptic observations of surface magnetic fields of low-mass stars. This led the stellar astrophysics community to adopt modeling techniques that have been used in solar physics using solar magnetograms. However, many of these techniques have been neglected by the solar community due to their failure to reproduce solar observations. Nevertheless, some of these techniques are still used to simulate the coronae and winds of solar analogs. Here we present a comparative study between two MHD models for the solar corona and solar wind. The first type of model is a polytropic wind model, and the second is the physics-based AWSOM model. We show that while the AWSOM model consistently reproduces many solar observations, the polytropic model fails to reproduce many of them, and in the cases where it does, its solutions are unphysical. Our recommendation is that polytropic models, which are used to estimate mass-loss rates and other parameters of solar analogs, must first be calibrated with solar observations. Alternatively, these models can be calibrated with models that capture more detailed physics of the solar corona (such as the AWSOM model) and that can reproduce solar observations in a consistent manner. Without such a calibration, the results of the polytropic models cannot be validated, but they can be wrongly used by others.
Owocki, Stanley P.; Sundqvist, Jon O.
2018-03-01
We analyse recent 2D simulations of the non-linear evolution of the line-deshadowing instability (LDI) in hot-star winds, to quantify how the associated highly clumped density structure can lead to a `turbulent porosity' reduction in continuum absorption and/or scattering. The basic method is to examine the statistical variations of mass column as a function of path length, and fit these to analytic forms that lead to simple statistical scalings for the associated mean extinction. A key result is that one can characterize porosity effects on continuum transport in terms of a single `turbulent porosity length', found here to scale as H ≈ (fcl - 1)a, where fcl ≡ 〈ρ2〉/〈ρ〉2 is the clumping factor in density ρ, and a is the density autocorrelation length. For continuum absorption or scattering in an optically thick layer, we find the associated effective reduction in opacity scales as ˜ 1/√{1+τ_H}, where τH ≡ κρH is the local optical thickness of this porosity length. For these LDI simulations, the inferred porosity lengths are small, only about a couple per cent of the stellar radius, H ≈ 0.02R*. For continuum processes like bound-free absorption of X-rays that are only marginally optically thick throughout the full stellar wind, this implies τH ≪ 1, and thus that LDI-generated porosity should have little effect on X-ray transport in such winds. The formalism developed here could however be important for understanding the porous regulation of continuum-driven, super-Eddington outflows from luminous blue variables.
Correlation between photoeletron and photoion in ultrafast multichannel photoionization of Ar
International Nuclear Information System (INIS)
Itakura, R.; Fushitani, M.; Hishikawa, A.; Sako, T.
2015-01-01
We theoretically investigate coherent dynamics of ions created through ultrafast multichannel photoionization from a viewpoint of photoelectron-photoion correlation. The model calculation on single-photon ionization of Ar reveals that the coherent hole dynamics in Ar + associated with a superposition of the spin-orbit states 2 PJ (J = 3/2 and 1/2) can be identified by monitoring only the photoion created by a Fourier-transform limited extreme ultraviolet (EUV) pulse with the fs pulse duration, while the coherence is lost by a chirped EUV pulse. It is demonstrated that by coincidence detection of the photoelectron and photoion the coherent hole dynamics can be extracted even in the case of ionization by a chirped EUV pulse with the sufficiently wide bandwidth
An Extreme X-ray Disk Wind in the Black Hole Candidate IGR J17091-3624
King, A. L.; Miller, J. M.; Raymond, J.; Fabian, A. C.; Reynolds, C. S.; Kallman, T. R.; Maitra, D.; Cackett, E. M.; Rupen, M. P.
2012-01-01
Chandra spectroscopy of transient stellar-mass black holes in outburst has clearly revealed accretion disk winds in soft, disk-dominated states, in apparent anti-correlation with relativistic jets in low/hard states. These disk winds are observed to be highly ionized. dense. and to have typical velocities of approx 1000 km/s or less projected along our line of sight. Here. we present an analysis of two Chandra High Energy Transmission Grating spectra of the Galactic black hole candidate IGR J17091-3624 and contemporaneous EVLA radio observations. obtained in 2011. The second Chandra observation reveals an absorption line at 6.91+/-0.01 keV; associating this line with He-like Fe XXV requires a blue-shift of 9300(+500/-400) km/ s (0.03c. or the escape velocity at 1000 R(sub schw)). This projected outflow velocity is an order of magnitude higher than has previously been observed in stellar-mass black holes, and is broadly consistent with some of the fastest winds detected in active galactic nuclei. A potential feature at 7.32 keV, if due to Fe XXVI, would imply a velocity of approx 14600 km/s (0.05c), but this putative feature is marginal. Photoionization modeling suggests that the accretion disk wind in IGR J17091-3624 may originate within 43,300 Schwarzschild radii of the black hole, and may be expelling more gas than accretes. The contemporaneous EVLA observations strongly indicate that jet activity was indeed quenched at the time of our Chandra observations. We discuss the results in the context of disk winds, jets, and basic accretion disk physics in accreting black hole systems
Photoionization and Recombination
Nahar, Sultana N.
2000-01-01
Theoretically self-consistent calculations for photoionization and (e + ion) recombination are described. The same eigenfunction expansion for the ion is employed in coupled channel calculations for both processes, thus ensuring consistency between cross sections and rates. The theoretical treatment of (e + ion) recombination subsumes both the non-resonant recombination ("radiative recombination"), and the resonant recombination ("di-electronic recombination") processes in a unified scheme. In addition to the total, unified recombination rates, level-specific recombination rates and photoionization cross sections are obtained for a large number of atomic levels. Both relativistic Breit-Pauli, and non-relativistic LS coupling, calculations are carried out in the close coupling approximation using the R-matrix method. Although the calculations are computationally intensive, they yield nearly all photoionization and recombination parameters needed for astrophysical photoionization models with higher precision than hitherto possible, estimated at about 10-20% from comparison with experimentally available data (including experimentally derived DR rates). Results are electronically available for over 40 atoms and ions. Photoionization and recombination of He-, and Li-like C and Fe are described for X-ray modeling. The unified method yields total and complete (e+ion) recombination rate coefficients, that can not otherwise be obtained theoretically or experimentally.
International Nuclear Information System (INIS)
Ovchinnikov, O.; Schlachter, F.
2003-01-01
Photoionization of Fe3+ ions was studied for the first time using synchrotron radiation from the Advanced Light Source (ALS) and the merged-beams technique. Fe3+ ions were successfully produced using ferrocene in an electron cyclotron resonance ion source (ECR). The measured yield of Fe4+ photoions as a function of photon energy revealed the presence of resonances that correspond to excitation of autoionizing states. These resonances are superimposed upon the photoion yield produced by direct photoionization, which is a smooth, slowly decreasing function of energy. The spectra for the photoionization of Fe3+ will be analyzed and compared with theory. The data collected will also serve to test models for the propagation of light through ionized matter.
Optogalvanic photoionization spectroscopy
International Nuclear Information System (INIS)
Levesque, S.; Gagne, J.-M.; Babin, F.
1997-01-01
This paper presents, for the first time, a systematic study of an optogalvanic method for photoionization spectroscopy. The method is particularly attractive for refractory and complex atoms, such as lanthanides and actinides. The relevant characteristics of the hollow cathode discharges used for this study are discussed in detail, along with the experimental protocol for this spectroscopic method. The rapid optogalvanic effect, which results solely from photoionization, is also described. Finally, we present as an example of the application of this method, a table containing some of the recorded uranium photoionization lines in the 16 300-20 500 cm -1 range, along with typical samples of the uranium single-colour photoionization spectrum recorded using the rapid optogalvanic technique. A brief discussion of the sensitivity of the rapid optogalvanic effect is also presented. It appears that the rapid optogalvanic effect is very effective in the detection of highly excited levels. This technique permitted the observation of many new single-colour resonant ionization uranium lines. (Author)
Photoionization effects in ionization fronts
International Nuclear Information System (INIS)
Arrayas, Manuel; Fontelos, Marco A; Trueba, Jose L
2006-01-01
In this paper we study the effects of photoionization processes on the propagation of both negative and positive ionization fronts in streamer discharge. We show that negative fronts accelerate in the presence of photoionization events. The appearance and propagation of positive ionization fronts travelling with constant velocity is explained as the result of the combined effects of photoionization and electron diffusion. The photoionization range plays an important role in the selection of the velocity of the ionization front as we show in this work
Photoionization effects in ionization fronts
Energy Technology Data Exchange (ETDEWEB)
Arrayas, Manuel [Departamento de Electromagnetismo, Universidad Rey Juan Carlos, Tulipan s/n, 28933 Mostoles, Madrid (Spain); Fontelos, Marco A [Departamento de Matematicas, Instituto de Matematicas y Fisica Fundamental, Consejo Superior de Investigaciones CientIficas, C/Serrano 123, 28006 Madrid (Spain); Trueba, Jose L [Departamento de Electromagnetismo, Universidad Rey Juan Carlos, Tulipan s/n, 28933 Mostoles, Madrid (Spain)
2006-12-21
In this paper we study the effects of photoionization processes on the propagation of both negative and positive ionization fronts in streamer discharge. We show that negative fronts accelerate in the presence of photoionization events. The appearance and propagation of positive ionization fronts travelling with constant velocity is explained as the result of the combined effects of photoionization and electron diffusion. The photoionization range plays an important role in the selection of the velocity of the ionization front as we show in this work.
Compact Starburst Galaxies with Fast Outflows: Spatially Resolved Stellar Mass Profiles
Gottlieb, Sophia; Diamond-Stanic, Aleksandar; Lipscomb, Charles; Ohene, Senyo; Rines, Josh; Moustakas, John; Sell, Paul; Tremonti, Christy; Coil, Alison; Rudnick, Gregory; Hickox, Ryan C.; Geach, James; Kepley, Amanda
2018-01-01
Powerful galactic winds driven by stellar feedback and black hole accretion are thought to play an important role in regulating star formation in galaxies. In particular, strong stellar feedback from supernovae, stellar winds, radiation pressure, and cosmic rays is required by simulations of star-forming galaxies to prevent the vast majority of baryons from cooling and collapsing to form stars. However, it remains unclear whether these stellar processes play a significant role in expelling gas and shutting down star formation in massive progenitors of quiescent galaxies. What are the limits of stellar feedback? We present multi-band photometry with HST/WFC3 (F475W, F814W, F160W) for a dozen compact starburst galaxies at z~0.6 with half-light radii that suggest incredibly large central escape velocities. These massive galaxies are driving fast (>1000 km/s) outflows that have been previously attributed to stellar feedback associated with the compact (r~100 pc) starburst. But how compact is the stellar mass? In the context of the stellar feedback hypothesis, it is unclear whether these fast outflows are being driven at velocities comparable to the escape velocity of an incredibly dense stellar system (as predicted by some models of radiation-pressure winds) or at velocities that exceed the central escape velocity by large factor. Our spatially resolved measurements with HST show that the stellar mass is more extended than the light, and this requires that the physical mechanism responsible for driving the winds must be able to launch gas at velocities that are factors of 5-10 beyond the central escape velocity.
Photoion mass spectroscopy and valence photoionization of hypoxanthine, xanthine and caffeine
Energy Technology Data Exchange (ETDEWEB)
Feyer, Vitaliy, E-mail: vitaliy.feyer@elettra.trieste.it [Sincrotrone Trieste, in Area Science Park, I-34012 Basovizza (Trieste) (Italy); Plekan, Oksana [Sincrotrone Trieste, in Area Science Park, I-34012 Basovizza (Trieste) (Italy)] [Institute of Electron Physics, 21 Universitetska St., 88017 Uzhgorod (Ukraine); Richter, Robert [Sincrotrone Trieste, in Area Science Park, I-34012 Basovizza (Trieste) (Italy); Coreno, Marcello [CNR-IMIP, Area della Ricerca di Roma 1, CP10, I-00016 Monterotondo Scalo (Italy)] [CNR-Laboratorio Nazionale TASC-INFM, I-34012 Basovizza (Trieste) (Italy); Prince, Kevin C. [Sincrotrone Trieste, in Area Science Park, I-34012 Basovizza (Trieste) (Italy)] [CNR-Laboratorio Nazionale TASC-INFM, I-34012 Basovizza (Trieste) (Italy)
2009-03-30
Photoionization mass spectra of hypoxanthine, xanthine and caffeine were measured using the photoelectron-photoion coincidence technique and noble gas resonance radiation at energies from 8.4 to 21.2 eV for ionization. The fragmentation patterns for these compounds show that hydrogen cyanide is the main neutral loss species at higher photon energies, while photoionization below 16.67 eV led predominantly to the parent ion. The valence photoelectron spectra of this family of molecules were measured over an extended energy range, including the inner C, N and O 2s valence orbitals. The observed ion fragments were related to ionization of the valence orbitals.
Energy Technology Data Exchange (ETDEWEB)
Germann, Matthias; Willitsch, Stefan, E-mail: stefan.willitsch@unibas.ch [Department of Chemistry, University of Basel, Klingelbergstrasse 80, 4056 Basel (Switzerland)
2016-07-28
We develop a model for predicting fine- and hyperfine intensities in the direct photoionization of molecules based on the separability of electron and nuclear spin states from vibrational-electronic states. Using spherical tensor algebra, we derive highly symmetrized forms of the squared photoionization dipole matrix elements from which we derive the salient selection and propensity rules for fine- and hyperfine resolved photoionizing transitions. Our theoretical results are validated by the analysis of the fine-structure resolved photoelectron spectrum of O{sub 2} reported by Palm and Merkt [Phys. Rev. Lett. 81, 1385 (1998)] and are used for predicting hyperfine populations of molecular ions produced by photoionization.
Germann, Matthias; Willitsch, Stefan
2016-07-28
We develop a model for predicting fine- and hyperfine intensities in the direct photoionization of molecules based on the separability of electron and nuclear spin states from vibrational-electronic states. Using spherical tensor algebra, we derive highly symmetrized forms of the squared photoionization dipole matrix elements from which we derive the salient selection and propensity rules for fine- and hyperfine resolved photoionizing transitions. Our theoretical results are validated by the analysis of the fine-structure resolved photoelectron spectrum of O2 reported by Palm and Merkt [Phys. Rev. Lett. 81, 1385 (1998)] and are used for predicting hyperfine populations of molecular ions produced by photoionization.
Photoionization and molecular structure
International Nuclear Information System (INIS)
Palma, A.
1983-01-01
A presentation is here given of the theoretical work on photoionization and molecular structure carried out by the author and coworkers. The implications of the photoionization process on the molecular geometry are emphasized. In particular, the ionization effect on deep orbitals is considered and it is shown that, contrary to traditional thinking, these orbitals have relevant effects on the molecular geometry. The problem of calculating photoionization relative intensities for the full spectrum is also considered, and the results of the present model are compared with experimental and other theoretical results. (author)
XMM-Newton X-ray observations of γ2 Velorum (WC8 + O7.5III)
International Nuclear Information System (INIS)
Raassen, A.J.J.; Mewe, R.; Hucht, K.A. van der; Schmutz, W.; Schild, H.; Dumm, T.; Guedel, M.; Audard, M.; Leutenegger, M.A.; Skinner, S.L.
2004-01-01
The spectrum of the binary system γ 2 Velorum (WC8 + O7.5III) has been observed with RGS and EPIC-MOS aboard XMM-Newton. The system shows a 'high state' when the O-star is between the Wolf-Rayet star and the observer (near periastron) and a 'low state' when most of the spectrum is absorbed by the dense stellar wind of the Wolf-Rayet star (near apastron). The spectrum has been model-led by a 4-T plasma, using SPEX. The absorption affects the hot temperature component (kT = 1.5 keV) that is formed by the collision of the Wolf-Rayet wind and the O-star wind, and the second hot component (kT 0.65 keV) for which the origin is still unclear. Part of the spectrum is not sensitive to the absorption by the stellar wind. This concerns a low-temperature component (kT = 0.23 keV) and features that are produced by plasma that has been photoionized by X-ray radiation from the hot component. In the RGS spectrum features of Radiative Recombination Continua (RRC) of C VI and C V of this photoionized plasma are detected
International Nuclear Information System (INIS)
Johnson, Mark
2001-01-01
The Gordon Research Conference on Photoions, Photoionization and Photodetachment was held at Williams College, Williamstown, Massachusetts, July 8-13, 2001. The 72 conference attendees represented the spectrum of endeavor in this field, coming from academia, industry, and government laboratories, and including US and foreign scientists, senior researchers, young investigators, and students. Emphasis was placed on current unpublished research and discussion of the future target areas in this field. There was a conscious effort to stimulate discussion about the key issues in the field today. Time for formal presentations was limited. Sessions included the following topics: Vibrational structure, Time resolved studies: nuclear wavepackets, Valence photoionization, Clusters and networks, Resonance structures and decay mechanisms, Ultrafast photoionization, Threshold photoionization, Molecule fixed properties, and Collisional phenomena
Engineering aspects of compact stellarators
International Nuclear Information System (INIS)
Nelson, B.E.; Benson, R.D.; Brooks, A.
2003-01-01
Compact stellarators could combine the good confinement and high beta of a tokamak with the inherently steady state, disruption-free characteristics of a stellarator. Two U.S. compact stellarator facilities are now in the conceptual design phase: the National Compact Stellarator Experiment (NCSX) and the Quasi- Poloidal Stellarator (QPS). NCSX has a major radius of 1.4 m and a toroidal field up to 2 T. The primary feature of both NCSX and QPS is the set of modular coils that provide the basic magnetic configuration. These coils represent a major engineering challenge due to the complex shape, precise geometric accuracy, and high current density of the windings. The winding geometry is too complex for conventional hollow copper conductor construction. Instead, the modular coils will be wound with flexible, multi strand cable conductor that has been compacted to a 75% copper packing fraction. Inside the NCSX coil set and surrounding the plasma is a highly contoured vacuum vessel. The vessel consists of three identical, 120 deg. segments that are bolted together at double sealed joints. The QPS device has a major radius of 0.9 m, a toroidal field of 1 T, and an aspect ratio of only 2.7. Instead of an internal vacuum vessel, the QPS modular coils will operate in an external vacuum tank. (author)
A spectroscopic search for colliding stellar winds in O-type close binary systems. IV - Iota Orionis
Gies, Douglas R.; Wiggs, Michael S.; Bagnuolo, William G., Jr.
1993-01-01
We present H-alpha and He I 6678 A line profiles for the eccentric orbit binary Iota Ori. We have applied a tomography algorithm which uses the established orbital velocity curves and intensity ratio to reconstruct the spectral line profiles for each star. The He I profiles appear as pure photospheric lines, and H-alpha shows variable emission in the line core throughout the orbit (which is typical of O giants) and in the blue wing near periastron passage. We show that the blue wing emission is consistent with an origin between the stars which probably results from a dramatic focusing of the primary's stellar wind at periastron. We also present IUE archival spectra of the UV wind lines N V 1240 A and C IV 1550 A.
Photoionization and dissociative photoionization study of HFC-152a using synchrotron radiation
International Nuclear Information System (INIS)
Huang Chaoqun; Wei Lixia; Yang Bin; Yang Rui; Wang Sisheng; Shan Xiaobin; Qi Fei; Zhang Yunwu; Sheng Liusi; Hao Liqing; Zhou Shikang; Wang Zhenya
2006-01-01
Photoionization and dissociative photoionization of HFC-152a have been studied using synchrotron radiation and a reflection time-of-flight mass spectrometry (RTOF-MS). The ionization energy of parent molecule (11.94 ± 0.04 eV) and appearance potentials of various fragment ions have been determined by measuring their photoionization efficiency curves. Energies, symmetry point groups and ground electronic states of neutrals and cations of parent and its fragments have been calculated using GAUSSIAN-03 program with the G3 method. According to the theoretical and experimental results, some dissociation channels and their dissociation energies of CH 3 CHF 2 + have been analyzed. (authors)
Photoionization of Co+ and electron-impact excitation of Co2 + using the Dirac R-matrix method
Tyndall, N. B.; Ramsbottom, C. A.; Ballance, C. P.; Hibbert, A.
2016-11-01
Modelling of massive stars and supernovae (SNe) plays a crucial role in understanding galaxies. From this modelling we can derive fundamental constraints on stellar evolution, mass-loss processes, mixing, and the products of nucleosynthesis. Proper account must be taken of all important processes that populate and depopulate the levels (collisional excitation, de-excitation, ionization, recombination, photoionization, bound-bound processes). For the analysis of Type Ia SNe and core collapse SNe (Types Ib, Ic and II) Fe group elements are particularly important. Unfortunately little data is currently available and most noticeably absent are the photoionization cross-sections for the Fe-peaks which have high abundances in SNe. Important interactions for both photoionization and electron-impact excitation are calculated using the relativistic Dirac atomic R-matrix codes (DARC) for low-ionization stages of Cobalt. All results are calculated up to photon energies of 45 eV and electron energies up to 20 eV. The wavefunction representation of Co III has been generated using GRASP0 by including the dominant 3d7, 3d6[4s, 4p], 3p43d9 and 3p63d9 configurations, resulting in 292 fine structure levels. Electron-impact collision strengths and Maxwellian averaged effective collision strengths across a wide range of astrophysically relevant temperatures are computed for Co III. In addition, statistically weighted level-resolved ground and metastable photoionization cross-sections are presented for Co II and compared directly with existing work.
International Nuclear Information System (INIS)
Zhao, Yujie; Cao, Maoqi; Li, Yuquan; Shan, Xiaobin; Liu, Fuyi; Sheng, Liusi; Li, Li; Liu, Wanfang
2014-01-01
Highlights: • The high resolution photoionization spectrum of carbon monoxide has been investigated using tunable synchrotron radiation. • This work has investigated comprehensively almost all kinds of photo excitation processes of CO in wide photon region. • The mechanisms of photoionization and dissociative photoionization of CO have been researched in detail. - Abstract: The vacuum-ultraviolet photoionization and dissociative photoionization of carbon monoxide in a region 14–38 eV have been investigated with time-of-flight (TOF) photoionization mass spectrometry (PIMS) using tunable synchrotron radiation (SR). The adiabatic ionization energy (IE) of carbon monoxide and appearance energies (AE) for its fragment ions in different states are determined by measurements of photoionization efficiency spectra (PIES). Ab initio calculations have been performed to investigate the reaction mechanism of dissociative photoionization of carbon monoxide. On the basis of experimental and predicted theoretical results, the mechanisms of photoionization and dissociative photoionization of molecular CO are discussed, and sixteen dissociative photoionization processes are proposed. The equilibrium geometries and harmonic vibrational frequencies of CO molecule, and its parent cation were calculated by using MP2 (full) method. The differences of configurations between them are also discussed on the basis of theoretical calculations. According to our results, the experimental IE of CO molecule, and dissociation energies (E d ) of possible dissociative channels are in reasonable agreement with the calculated values of the proposed photodissociation channels
Scientists Find X Rays from Stellar Winds That May Play Significant Role in Galactic Evolution
2001-09-01
Colorful star-forming regions that have captivated stargazers since the advent of the telescope 400 years ago contain gas thousands of times more energetic than previously recognized, powered by colliding stellar winds. This multimillion-degree gas radiated as X rays is one of the long-sought sources of energy and elements in the Milky Way galaxy's interstellar medium. A team led by Leisa Townsley, a senior research associate in astronomy and astrophysics at Penn State University, uncovered this wind phenomenon in the Rosette Nebula, a stellar nursery. With the Chandra X-ray Observatory, the team found that the most massive stars in the nebula produce winds that slam into each other, create violent shocks, and infuse the region with 6-million-degree gas. The findings are presented in Washington, D.C., today at a conference entitled "Two Years of Science with Chandra." "A ghostly glow of diffuse X-ray emission pervades the Rosette Nebula and perhaps many other similar star-forming regions throughout the Galaxy," said Townsley. "We now have a new view of the engine lighting the beautiful Rosette Nebula and new evidence for how the interstellar medium may be energized." Townsley and her colleagues created a striking X-ray panorama of the Rosette Molecular Cloud from four images with Chandra's Advanced CCD Imaging Spectrometer. This is a swath of the sky nearly 100 light years across sprayed with hundreds of X-ray-emitting young stars. In one corner of the Rosette Molecular Cloud lies the Rosette Nebula, called an "H II region" because the hydrogen gas there has been stripped of its electrons due to the strong ultraviolet radiation from its young stars. This region, about 5,000 light years away in the constellation Monoceros, the Unicorn, has long been a favorite among amateur astronomers. The wispy, colorful display is visible with small telescopes. The Chandra survey reveals, for the first time, 6-million-degree gas at the center of the Rosette Nebula, occupying a
Energy Technology Data Exchange (ETDEWEB)
Shaikhislamov, I. F.; Prokopov, P. A.; Berezutsky, A. G.; Zakharov, Yu. P.; Posukh, V. G. [Institute of Laser Physics SB RAS, Novosibirsk (Russian Federation); Khodachenko, M. L.; Lammer, H.; Kislyakova, K. G.; Fossati, L. [Space Research Institute, Austrian Acad. Sci., Graz (Austria); Johnstone, C. P., E-mail: maxim.khodachenko@oeaw.ac.at [Department of Astrophysics, University of Vienna, Vienna (Austria)
2016-12-01
The interaction of escaping the upper atmosphere of a hydrogen-rich non-magnetized analog of HD 209458b with a stellar wind (SW) of its host G-type star at different orbital distances is simulated with a 2D axisymmetric multi-fluid hydrodynamic (HD) model. A realistic Sun-like spectrum of X-ray and ultraviolet radiation, which ionizes and heats the planetary atmosphere, together with hydrogen photochemistry, as well as stellar-planetary tidal interaction are taken into account to generate self-consistently an atmospheric HD outflow. Two different regimes of the planetary and SW interaction have been modeled. These are: (1) the “ captured by the star ” regime, when the tidal force and pressure gradient drive the planetary material beyond the Roche lobe toward the star, and (2) the “ blown by the wind ” regime, when sufficiently strong SW confines the escaping planetary atmosphere and channels it into the tail. The model simulates in detail the HD interaction between the planetary atoms, protons and the SW, as well as the production of energetic neutral atoms (ENAs) around the planet due to charge exchange between planetary atoms and stellar protons. The revealed location and shape of the ENA cloud, either as a paraboloid shell between the ionopause and bowshock (for the “ blown by the wind ” regime), or a turbulent layer at the contact boundary between the planetary stream and SW (for the “ captured by the star ” regime) are of importance for the interpretation of Ly α absorption features in exoplanetary transit spectra and characterization of the plasma environments.
International Nuclear Information System (INIS)
Shaikhislamov, I. F.; Prokopov, P. A.; Berezutsky, A. G.; Zakharov, Yu. P.; Posukh, V. G.; Khodachenko, M. L.; Lammer, H.; Kislyakova, K. G.; Fossati, L.; Johnstone, C. P.
2016-01-01
The interaction of escaping the upper atmosphere of a hydrogen-rich non-magnetized analog of HD 209458b with a stellar wind (SW) of its host G-type star at different orbital distances is simulated with a 2D axisymmetric multi-fluid hydrodynamic (HD) model. A realistic Sun-like spectrum of X-ray and ultraviolet radiation, which ionizes and heats the planetary atmosphere, together with hydrogen photochemistry, as well as stellar-planetary tidal interaction are taken into account to generate self-consistently an atmospheric HD outflow. Two different regimes of the planetary and SW interaction have been modeled. These are: (1) the “ captured by the star ” regime, when the tidal force and pressure gradient drive the planetary material beyond the Roche lobe toward the star, and (2) the “ blown by the wind ” regime, when sufficiently strong SW confines the escaping planetary atmosphere and channels it into the tail. The model simulates in detail the HD interaction between the planetary atoms, protons and the SW, as well as the production of energetic neutral atoms (ENAs) around the planet due to charge exchange between planetary atoms and stellar protons. The revealed location and shape of the ENA cloud, either as a paraboloid shell between the ionopause and bowshock (for the “ blown by the wind ” regime), or a turbulent layer at the contact boundary between the planetary stream and SW (for the “ captured by the star ” regime) are of importance for the interpretation of Ly α absorption features in exoplanetary transit spectra and characterization of the plasma environments.
The Effects of Stellar Dynamics on the Evolution of Young, Dense Stellar Systems
Belkus, H.; van Bever, J.; Vanbeveren, D.
In this paper, we report on first results of a project in Brussels in which we study the effects of stellar dynamics on the evolution of young dense stellar systems using 3 decades of expertise in massive-star evolution and our population (number and spectral) synthesis code. We highlight an unconventionally formed object scenario (UFO-scenario) for Wolf Rayet binaries and study the effects of a luminous blue variable-type instability wind mass-loss formalism on the formation of intermediate-mass black holes.
Photoionization of atoms and molecules
International Nuclear Information System (INIS)
Samson, J.A.R.
1976-01-01
A literature review on the present state of knowledge in photoionization is presented. Various experimental techniques that have been developed to study photoionization, such as fluorescence and photoelectron spectroscopy, mass spectroscopy, are examined. Various atoms and molecules were chosen to illustrate these techniques, specifically helium and xenon atoms and hydrogen molecules. Specialized photoionization such as in positive and negative ions, excited states, and free radicals is also treated. Absorption cross sections and ionization potentials are also discussed
Photoionization at relativistic energies
International Nuclear Information System (INIS)
Ionescu, D.C.; Technische Univ. Dresden; Soerensen, A.H.; Belkacem, A.
2000-11-01
At MeV energies and beyond the inner-shell vacancy production cross section associated with the photoelectric and Compton effect decrease with increasing photon energy. However, when the photon energy exceeds twice the rest energy of the electron, ionization of a bound electron may be catalyzed by the creation of an electron-positron pair. Distinctly different from all other known mechanisms for inner-shell vacancy production by photons, we show that the cross section for this ''vacuum-assisted photoionization'' increases with increasing photon energy and then saturates. As a main result, we predict that vacuum-assisted photoionization will dominate the other known photoionization mechanisms in the highly relativistic energy regime. (orig.)
Many body perturbation calculations of photoionization
International Nuclear Information System (INIS)
Kelly, H.P.
1979-01-01
The application of many body perturbation theory to the calculation of atomic photoionization cross sections is reviewed. The choice of appropriate potential for the single-particle state is discussed and results are presented for several atoms including resonance structure. In addition to single photoionization, the process of double photoionization is considered and is found to be significant. (Auth.)
Otsuka, Masaaki; Ueta, Toshiya; van Hoof, Peter A M; Sahai, Raghvendra; Aleman, Isabel; Zijlstra, Albert A; Chu, You-Hua; Villaver, Eva; Leal-Ferreira, Marcelo L; Kastner, Joel; Szczerba, Ryszard; Exter, Katrina M
2017-08-01
We perform a comprehensive analysis of the planetary nebula (PN) NGC 6781 to investigate the physical conditions of each of its ionized, atomic, and molecular gas and dust components and the object's evolution, based on panchromatic observational data ranging from UV to radio. Empirical nebular elemental abundances, compared with theoretical predictions via nucleosynthesis models of asymptotic giant branch (AGB) stars, indicate that the progenitor is a solar-metallicity, 2.25-3.0 M ⊙ initial-mass star. We derive the best-fit distance of 0.46 kpc by fitting the stellar luminosity (as a function of the distance and effective temperature of the central star) with the adopted post-AGB evolutionary tracks. Our excitation energy diagram analysis indicates high-excitation temperatures in the photodissociation region (PDR) beyond the ionized part of the nebula, suggesting extra heating by shock interactions between the slow AGB wind and the fast PN wind. Through iterative fitting using the Cloudy code with empirically derived constraints, we find the best-fit dusty photoionization model of the object that would inclusively reproduce all of the adopted panchromatic observational data. The estimated total gas mass (0.41 M ⊙ ) corresponds to the mass ejected during the last AGB thermal pulse event predicted for a 2.5 M ⊙ initial-mass star. A significant fraction of the total mass (about 70%) is found to exist in the PDR, demonstrating the critical importance of the PDR in PNe that are generally recognized as the hallmark of ionized/H + regions.
Energy Technology Data Exchange (ETDEWEB)
Klaus Muller-Dethefs
2009-03-31
This conference brings together scientists interested in a range of basic phenomena linked to the ejection and scattering of electrons from atoms, molecules, clusters, liquids and solids by absorption of light. Photoionization, a highly sensitive probe of both structure and dynamics, can range from perturbative single-photon processes to strong-field highly non-perturbative interactions. It is responsible for the formation and destruction of molecules in astrophysical and plasma environments and successfully used in advanced analytical techniques. Positive ions, which can be produced and studied most effectively using photoionization, are the major components of all plasmas, vital constituents of flames and important intermediates in many chemical reactions. Negative ions are significant as transient species and, when photodetached, the corresponding neutral species often undergoes remarkable, otherwise non-observable, dynamics. The scope of the meeting spans from novel observations in atomic and molecular physics, such as Coulomb Crystals, highly excited states and cold Rydberg plasmas, to novel energy resolved or ultrafast time-resolved experiments, photoionization in strong laser fields, theoretical method development for electron scattering, photoionization and photodetachment and more complex phenomena such as charge transfer and DNA and protein conductivity, important for biological and analytical applications.
Excited-state molecular photoionization dynamics
International Nuclear Information System (INIS)
Pratt, S.T.
1995-01-01
This review presents a survey of work using resonance-enhanced multiphoton ionization and double-resonance techniques to study excited-state photoionization dynamics in molecules. These techniques routinely provide detail and precision that are difficult to achieve in single-photon ionization from the ground state. The review not only emphasizes new aspects of photoionization revealed in the excited-state experiments but also shows how the excited-state techniques can provide textbook illustrations of some fundamental mechanisms in molecular photoionization dynamics. Most of the examples are confined to diatomic molecules. (author)
Photoionization Efficiencies of Five Polycyclic Aromatic Hydrocarbons.
Johansson, K Olof; Campbell, Matthew F; Elvati, Paolo; Schrader, Paul E; Zádor, Judit; Richards-Henderson, Nicole K; Wilson, Kevin R; Violi, Angela; Michelsen, Hope A
2017-06-15
We have measured photoionization-efficiency curves for pyrene, fluoranthene, chrysene, perylene, and coronene in the photon energy range of 7.5-10.2 eV and derived their photoionization cross-section curves in this energy range. All measurements were performed using tunable vacuum ultraviolet (VUV) radiation generated at the Advanced Light Source synchrotron at Lawrence Berkeley National Laboratory. The VUV radiation was used for photoionization, and detection was performed using a time-of-flight mass spectrometer. We measured the photoionization efficiency of 2,5-dimethylfuran simultaneously with those of pyrene, fluoranthene, chrysene, perylene, and coronene to obtain references of the photon flux during each measurement from the known photoionization cross-section curve of 2,5-dimethylfuran.
International Nuclear Information System (INIS)
Shah, M.L.; Sahoo, A.C.; Pulhani, A.K.; Gupta, G.P.; Dikshit, B.; Bhatia, M.S.; Suri, B.M.
2014-01-01
Laser-induced photoionization and fluorescence signals were simultaneously observed in atomic samarium using Nd:YAG-pumped dye lasers. Two-color, three-photon photoionization and two-color fluorescence signals were recorded simultaneously as a function of the second-step laser power for two photoionization pathways. The density matrix formalism has been employed to analyze these signals. Two-color laser-induced fluorescence signal depends on the laser powers used for the first and second-step transitions as well as the first and second-step transition probability whereas two-color, three-photon photoionization signal depends on the third-step transition cross-section at the second-step laser wavelength along with the laser powers and transition probability for the first and second-step transitions. Two-color laser-induced fluorescence was used to measure the second-step transition probability. The second-step transition probability obtained was used to infer the photoionization cross-section. Thus, the methodology combining two-color, three-photon photoionization and two-color fluorescence signals in a single experiment has been established for the first time to measure the second-step transition probability as well as the photoionization cross-section. - Highlights: • Laser-induced photoionization and fluorescence signals have been simultaneously observed. • The density matrix formalism has been employed to analyze these signals. • Two-color laser-induced fluorescence was used to measure the second-step transition probability. • The second-step transition probability obtained was used to infer the photoionization cross-section. • Transition probability and photoionization cross-section have been measured in a single experiment
International Nuclear Information System (INIS)
Poe, C.H.; Owocki, S.P.; Castor, J.I.
1990-01-01
The steady state solution topology for absorption line-driven flows is investigated for the condition that the Sobolev approximation is not used to compute the line force. The solution topology near the sonic point is of the nodal type with two positive slope solutions. The shallower of these slopes applies to reasonable lower boundary conditions and realistic ion thermal speed v(th) and to the Sobolev limit of zero of the usual Castor, Abbott, and Klein model. At finite v(th), this solution consists of a family of very similar solutions converging on the sonic point. It is concluded that a non-Sobolev, absorption line-driven flow with a realistic values of v(th) has no uniquely defined steady state. To the extent that a pure absorption model of the outflow of stellar winds is applicable, radiatively driven winds should be intrinsically variable. 34 refs
Density-dependent expressions for photoionization cross-sections
International Nuclear Information System (INIS)
Sun Weiguo; Ma Xiaoguang; Cheng Yansong
2004-01-01
Alternative expressions for photoionization cross-sections and dielectric influence functions are suggested to study the photoionization cross-sections of atoms in solid system. The basic picture is that the photoionization cross-section of atoms in a real system can be described as the coupling between quantum quantity (QQ) and classical quantity (CQ) parts. The QQ part represents the photoionization cross-sections of an isolated particle, while the CQ part may represent most of the important influence of the macroscopic effects (e.g., the interactions of all surrounding polarized particles, and the dielectric property, etc.) on the photoionization cross-sections. The applications to the barium system show that the number-density-dependent new photoionization formula not only obtains the same cross-sections as those from the first order approximation for ideal gas, but also can generate the cross-sections for solid barium by transforming those of ideal gas of the same species using the dielectric influence function
Density-dependent expressions for photoionization cross-sections
Energy Technology Data Exchange (ETDEWEB)
Sun Weiguo; Ma Xiaoguang; Cheng Yansong
2004-06-07
Alternative expressions for photoionization cross-sections and dielectric influence functions are suggested to study the photoionization cross-sections of atoms in solid system. The basic picture is that the photoionization cross-section of atoms in a real system can be described as the coupling between quantum quantity (QQ) and classical quantity (CQ) parts. The QQ part represents the photoionization cross-sections of an isolated particle, while the CQ part may represent most of the important influence of the macroscopic effects (e.g., the interactions of all surrounding polarized particles, and the dielectric property, etc.) on the photoionization cross-sections. The applications to the barium system show that the number-density-dependent new photoionization formula not only obtains the same cross-sections as those from the first order approximation for ideal gas, but also can generate the cross-sections for solid barium by transforming those of ideal gas of the same species using the dielectric influence function.
Photoionization studies with molecular beams
International Nuclear Information System (INIS)
Ng, C.Y.
1976-09-01
A molecular beam photoionization apparatus which combines the advantages of both the molecular beam method with photoionization mass spectrometry has been designed and constructed for carrying out some unique photoionization experiments. Rotational cooling during the supersonic expansion has resulted in high resolution photoionization efficiency curves for NO, ICl, C 2 H 2 and CH 3 I. The analysis of these spectra has yielded ionization potentials for these molecules to an accuracy of +- 3 MeV. Detailed autoionization structures were also resolved. This allows the investigation of the selection rules for autoionization, and the identification of the Rydberg series which converge to the excited states of the molecular ions. The degree of relaxation for thermally populated excited states has been examined using NO and ICl as examples. As a result of adiabatic cooling, a small percentage of dimers is also formed during the expansion. The photoionization efficiency curves for (NO) 2 , ArICl, Ar 2 , Kr 2 and Xe 2 have been obtained near the thresholds. Using the known dissociation energies of the (NO) 2 , Ar 2 , Kr 2 and Xe 2 van der Waals molecules, the corresponding dissociation energies for NO-NO + , Ar 2 + , Kr 2 + , and Xe 2 + have been determined. The ionization mechanisms for this class of molecules are examined and discussed
Photoionization of the Buckminsterfullerene Cation.
Douix, Suzie; Duflot, Denis; Cubaynes, Denis; Bizau, Jean-Marc; Giuliani, Alexandre
2017-01-05
Photoionization of a buckminsterfullerene ion is investigated using an ion trap and a merged beam setup coupled to synchrotron radiation beamlines and compared to theoretical calculations. Absolute measurements derived from the ion trap experiment allow discrepancies concerning the photoionization cross section of C 60 + to be solved.
Rotational distributions of molecular photoions following resonant excitation
International Nuclear Information System (INIS)
Poliakoff, E.D.; Chan, J.C.K.; White, M.G.
1986-01-01
We demonstrate that the photoelectron energy mediates the rotational energy distribution of N + 2 ions created by photoionization, and conversely, that rotational energy determinations probe resonant excitation in molecular photoionization. Experimentally, this is accomplished by monitoring the dispersed fluorescence from N + 2 (B 2 Σ + /sub u/) photoions to determine their rotational energy distribution. These results demonstrate that while dipole selection rules constrain the total angular momentum of the electron--ion complex, the partitioning of angular momentum between the photoelectron and photoion depends on the photoejection dynamics. Implications for photoionization and electron impact ionizatin studies are discussed
Holzmeier, Fabian; Fischer, Ingo; Kiendl, Benjamin; Krueger, Anke; Bodi, Andras; Hemberger, Patrick
2016-04-07
We report the determination of the absolute photoionization cross section of cyclopropenylidene, c-C3H2, and the heat of formation of the C3H radical and ion derived by the dissociative ionization of the carbene. Vacuum ultraviolet (VUV) synchrotron radiation as provided by the Swiss Light Source and imaging photoelectron photoion coincidence (iPEPICO) were employed. Cyclopropenylidene was generated by pyrolysis of a quadricyclane precursor in a 1 : 1 ratio with benzene, which enabled us to derive the carbene's near threshold absolute photoionization cross section from the photoionization yield of the two pyrolysis products and the known cross section of benzene. The cross section at 9.5 eV, for example, was determined to be 4.5 ± 1.4 Mb. Upon dissociative ionization the carbene decomposes by hydrogen atom loss to the linear isomer of C3H(+). The appearance energy for this process was determined to be AE(0K)(c-C3H2; l-C3H(+)) = 13.67 ± 0.10 eV. The heat of formation of neutral and cationic C3H was derived from this value via a thermochemical cycle as Δ(f)H(0K)(C3H) = 725 ± 25 kJ mol(-1) and Δ(f)H(0K)(C3H(+)) = 1604 ± 19 kJ mol(-1), using a previously reported ionization energy of C3H.
Photoelectron photoion molecular beam spectroscopy
International Nuclear Information System (INIS)
Trevor, D.J.
1980-12-01
The use of supersonic molecular beams in photoionization mass spectroscopy and photoelectron spectroscopy to assist in the understanding of photoexcitation in the vacuum ultraviolet is described. Rotational relaxation and condensation due to supersonic expansion were shown to offer new possibilities for molecular photoionization studies. Molecular beam photoionization mass spectroscopy has been extended above 21 eV photon energy by the use of Stanford Synchrotron Radiation Laboratory (SSRL) facilities. Design considerations are discussed that have advanced the state-of-the-art in high resolution vuv photoelectron spectroscopy. To extend gas-phase studies to 160 eV photon energy, a windowless vuv-xuv beam line design is proposed
Laboratory studies of photoionized plasma related to astrophysics
International Nuclear Information System (INIS)
Yang Peiqiang; Wang Feilu; Zhao Gang
2011-01-01
Photoionized plasma is universal in astronomy and has great importance on account of its close relation to compact astrophysical objects such as black holes. Recently, with the development of high energy density lasers and Z-pinch facilities, it has become possible to simulate astronomical photoionized plasma in the laboratory. These experiments help us to benchmark and modify the photoionization models, and to understand the photoionization processes to diagnose related astronomical plasma environments. (authors)
International Nuclear Information System (INIS)
Pomphrey, N.; Berry, L.A.; Boozer, A.H.
2001-01-01
Experimental devices to study the physics of high-beta (β>∼4%), low aspect ratio (A<∼4.5) stellarator plasmas require coils that will produce plasmas satisfying a set of physics goals, provide experimental flexibility, and be practical to construct. In the course of designing a flexible coil set for the National Compact Stellarator Experiment, we have made several innovations that may be useful in future stellarator design efforts. These include: the use of Singular Value Decomposition methods for obtaining families of smooth current potentials on distant coil winding surfaces from which low current density solutions may be identified; the use of a Control Matrix Method for identifying which few of the many detailed elements of the stellarator boundary must be targeted if a coil set is to provide fields to control the essential physics of the plasma; the use of Genetic Algorithms for choosing an optimal set of discrete coils from a continuum of potential contours; the evaluation of alternate coil topologies for balancing the tradeoff between physics objective and engineering constraints; the development of a new coil optimization code for designing modular coils, and the identification of a 'natural' basis for describing current sheet distributions. (author)
Absolute photoionization cross-section of the methyl radical.
Taatjes, Craig A; Osborn, David L; Selby, Talitha M; Meloni, Giovanni; Fan, Haiyan; Pratt, Stephen T
2008-10-02
The absolute photoionization cross-section of the methyl radical has been measured using two completely independent methods. The CH3 photoionization cross-section was determined relative to that of acetone and methyl vinyl ketone at photon energies of 10.2 and 11.0 eV by using a pulsed laser-photolysis/time-resolved synchrotron photoionization mass spectrometry method. The time-resolved depletion of the acetone or methyl vinyl ketone precursor and the production of methyl radicals following 193 nm photolysis are monitored simultaneously by using time-resolved synchrotron photoionization mass spectrometry. Comparison of the initial methyl signal with the decrease in precursor signal, in combination with previously measured absolute photoionization cross-sections of the precursors, yields the absolute photoionization cross-section of the methyl radical; sigma(CH3)(10.2 eV) = (5.7 +/- 0.9) x 10(-18) cm(2) and sigma(CH3)(11.0 eV) = (6.0 +/- 2.0) x 10(-18) cm(2). The photoionization cross-section for vinyl radical determined by photolysis of methyl vinyl ketone is in good agreement with previous measurements. The methyl radical photoionization cross-section was also independently measured relative to that of the iodine atom by comparison of ionization signals from CH3 and I fragments following 266 nm photolysis of methyl iodide in a molecular-beam ion-imaging apparatus. These measurements gave a cross-section of (5.4 +/- 2.0) x 10(-18) cm(2) at 10.460 eV, (5.5 +/- 2.0) x 10(-18) cm(2) at 10.466 eV, and (4.9 +/- 2.0) x 10(-18) cm(2) at 10.471 eV. The measurements allow relative photoionization efficiency spectra of methyl radical to be placed on an absolute scale and will facilitate quantitative measurements of methyl concentrations by photoionization mass spectrometry.
Schwinger variational principle applied to molecular photoionization
International Nuclear Information System (INIS)
Smith, M.E.
1985-01-01
A method based upon the Schwinger variational principle was developed to study molecular photoionization and electron-molecule scattering. Exact static-exchange solutions to the equations for the continuum orbitals are obtained within the Hartree-Fock approximation; and from these cross sections and angular distributions are derived for both of the above processes. This method was applied to photoionization of the valence levels of three different systems. The first application of this method is a study of the photoionization of the valence levels of NO. Next, vibrationally resolved branching ratios and vibrational state-specific asymmetry parameters for photoionization of the 5sigma level of CO are presented. Finally, a study of the photoionization of the 5sigma level of CO absorbed on a nickel surface is reported. Approximating this system by the linear triatomic molecule NiCO leads to cross sections and angular distributions which are in good agreement with experimental data
Molecular Frame Reconstruction Using Time-Domain Photoionization Interferometry.
Marceau, Claude; Makhija, Varun; Platzer, Dominique; Naumov, A Yu; Corkum, P B; Stolow, Albert; Villeneuve, D M; Hockett, Paul
2017-08-25
Photoionization of molecular species is, essentially, a multipath interferometer with both experimentally controllable and intrinsic molecular characteristics. In this work, XUV photoionization of impulsively aligned molecular targets (N_{2}) is used to provide a time-domain route to "complete" photoionization experiments, in which the rotational wave packet controls the geometric part of the photoionization interferometer. The data obtained is sufficient to determine the magnitudes and phases of the ionization matrix elements for all observed channels, and to reconstruct molecular frame interferograms from lab frame measurements. In principle, this methodology provides a time-domain route to complete photoionization experiments and the molecular frame, which is generally applicable to any molecule (no prerequisites), for all energies and ionization channels.
Atmospheric pressure photoionization using tunable VUV synchrotron radiation
International Nuclear Information System (INIS)
Giuliani, A.; Giorgetta, J.-L.; Ricaud, J.-P.; Jamme, F.; Rouam, V.; Wien, F.; Laprévote, O.; Réfrégiers, M.
2012-01-01
Highlights: ► Coupling of an atmospheric pressure photoionization source with a vacuum ultra-violet (VUV) beamline. ► The set up allows photoionization up to 20 eV. ► Compared to classical atmospheric pressure photoionization (APPI), our set up offers spectral purity and tunability. ► Allows photoionization mass spectrometry on fragile and hard to vaporize molecules. - Abstract: We report here the first coupling of an atmospheric pressure photoionization (APPI) source with a synchrotron radiation beamline in the vacuum ultra-violet (VUV). A commercial APPI source of a QStar Pulsar i from AB Sciex was modified to receive photons from the DISCO beamline at the SOLEIL synchrotron radiation facility. Photons are delivered at atmospheric pressure in the 4–20 eV range. The advantages of this new set up, termed SR-APPI, over classical APPI are spectral purity and continuous tunability. The technique may also be used to perform tunable photoionization mass spectrometry on fragile compounds difficult to vaporize by classical methods.
Ayres, T. R.; Linsky, J. L.
1975-01-01
The formation of the Balmer-series member H-epsilon in the near-red wing of the Ca II H line is discussed for two cases: the sun (H-epsilon absorption profile) and Arcturus (H-epsilon emission profile). It is shown that although the H-epsilon source functions in both stars are dominated by the Balmer-continuum radiation field through photoionizations, the line-formation problems in the two stars are quantitatively different, owing to a substantial difference in the relative importance of the stellar chromosphere temperature inversion as compared with the stellar photosphere.
Photoionization studies with molecular beams
Energy Technology Data Exchange (ETDEWEB)
Ng, C.Y.
1976-09-01
A molecular beam photoionization apparatus which combines the advantages of both the molecular beam method with photoionization mass spectrometry has been designed and constructed for carrying out some unique photoionization experiments. Rotational cooling during the supersonic expansion has resulted in high resolution photoionization efficiency curves for NO, ICl, C/sub 2/H/sub 2/ and CH/sub 3/I. The analysis of these spectra has yielded ionization potentials for these molecules to an accuracy of +- 3 MeV. Detailed autoionization structures were also resolved. This allows the investigation of the selection rules for autoionization, and the identification of the Rydberg series which converge to the excited states of the molecular ions. The degree of relaxation for thermally populated excited states has been examined using NO and ICl as examples. As a result of adiabatic cooling, a small percentage of dimers is also formed during the expansion. The photoionization efficiency curves for (NO)/sub 2/, ArICl, Ar/sub 2/, Kr/sub 2/ and Xe/sub 2/ have been obtained near the thresholds. Using the known dissociation energies of the (NO)/sub 2/, Ar/sub 2/, Kr/sub 2/ and Xe/sub 2/ van der Waals molecules, the corresponding dissociation energies for NO-NO/sup +/, Ar/sub 2//sup +/, Kr/sub 2//sup +/, and Xe/sub 2//sup +/ have been determined. The ionization mechanisms for this class of molecules are examined and discussed.
Photoionization of H2O at high resolution
International Nuclear Information System (INIS)
Dehmer, P.M.; Chupka, W.A.
1978-01-01
The relative photoionization cross sections for the formation of H 2 O + , OH + , and H + from H 2 O were measured at high wavelength resolution using a 3-meter photoionization mass spectrometer equipped with a quadrupole mass flter and a 1-meter photoionization mass spectrometer equipped with a 12-inch radius, 60 0 sector magnetic mass spectrometer. Discrete structure in the parent ion photoionization efficiency curve is interpreted in terms of Rydberg series converging to excited states of the H 2 O + ion. 9 references
Highly Resolved Studies of Vacuum Ultraviolet Photoionization Dynamics
Kakar, Sandeep
We use measurements of dispersed fluorescence from electronically excited photoions to study fundamental aspects of intramolecular dynamics. Our experimental innovations make it possible to obtain highly resolved photoionization data that offer qualitative insights into molecular scattering. In particular, we obtain vibrationally resolved data to probe coupling between the electronic and nuclear degrees of freedom by studying the distribution of vibrational energy among photoions. Vibrationally resolved branching ratios are measured over a broad spectral range of excitation energy and their non-Franck-Condon behavior is used as a tool to investigate two diverse aspects of shape resonant photoionization. First, vibrational branching ratios are obtained for the SiF_4 5a _1^{-1} and CS_2 5sigma_{rm u} ^{-1} photoionization channels to help elucidate the microscopic aspects of shape resonant wavefunction for polyatomic molecules. It is shown that in such molecules the shape resonant wavefunction is not necessarily attributable to a specific bond in the molecule. Second, the multichannel aspect of shape resonant photoionization dynamics, reflected in continuum channel coupling, is investigated by obtaining vibrational branching ratios for the 2 sigma_{rm u}^{ -1} and 4sigma^{ -1} photoionization of the isoelectronic molecules N_2 and CO, respectively. These data indicate that effects of continuum coupling may be widespread. We also present the first set of rotationally resolved data over a wide energy range for the 2 sigma_{rm u}^{ -1} photoionization of N_2. These data probe the partitioning of the angular momentum between the photoelectron and photoion, and highlight the multicenter nature of the molecular potential. These case studies illustrate the utility of dispersed fluorescence measurements as a complement to photoelectron spectroscopy for obtaining highly resolved data for molecular photoionization. These measurements makes it possible to probe intrinsically
The role of photoionization in negative corona discharge
Directory of Open Access Journals (Sweden)
B. X. Lu
2016-09-01
Full Text Available The effect of photoionization on the negative corona discharge was simulated based on the needle to plane air gaps. The Trichel pulse, pulse train, electron density and the distribution of electric field will be discussed in this manuscript. Effect of photoionization on the magnitude and interval of the first pulse will be discussed for different applied voltages. It is demonstrated that the peak of the first pulse current could be weakened by photoionization and a critical voltage of the first pulse interval influenced by photoionization was given.
Stellar Winds and Dust Avalanches in the AU Mic Debris Disk
Energy Technology Data Exchange (ETDEWEB)
Chiang, Eugene; Fung, Jeffrey, E-mail: echiang@astro.berkeley.edu, E-mail: jeffrey.fung@berkeley.edu [Department of Astronomy, University of California at Berkeley, Campbell Hall, Berkeley, CA 94720-3411 (United States)
2017-10-10
We explain the fast-moving, ripple-like features in the edge-on debris disk orbiting the young M dwarf AU Mic. The bright features are clouds of submicron dust repelled by the host star’s wind. The clouds are produced by avalanches: radial outflows of dust that gain exponentially more mass as they shatter background disk particles in collisional chain reactions. The avalanches are triggered from a region a few au across—the “avalanche zone”—located on AU Mic’s primary “birth” ring at a true distance of ∼35 au from the star but at a projected distance more than a factor of 10 smaller: the avalanche zone sits directly along the line of sight to the star, on the side of the ring nearest Earth, launching clouds that disk rotation sends wholly to the southeast, as observed. The avalanche zone marks where the primary ring intersects a secondary ring of debris left by the catastrophic disruption of a progenitor up to Varuna in size, less than tens of thousands of years ago. Only where the rings intersect are particle collisions sufficiently violent to spawn the submicron dust needed to seed the avalanches. We show that this picture works quantitatively, reproducing the masses, sizes, and velocities of the observed escaping clouds. The Lorentz force exerted by the wind’s magnetic field, whose polarity reverses periodically according to the stellar magnetic cycle, promises to explain the observed vertical undulations. The timescale between avalanches, about 10 yr, might be set by time variability of the wind mass loss rate or, more speculatively, by some self-regulating limit cycle.
On the stability of bow shocks generated by red supergiants: the case of IRC -10414
Meyer, D. M.-A.; Gvaramadze, V. V.; Langer, N.; Mackey, J.; Boumis, P.; Mohamed, S.
2014-03-01
In this Letter, we explore the hypothesis that the smooth appearance of bow shocks around some red supergiants (RSGs) might be caused by the ionization of their winds by external sources of radiation. Our numerical simulations of the bow shock generated by IRC -10414 (the first-ever RSG with an optically detected bow shock) show that the ionization of the wind results in its acceleration by a factor of 2, which reduces the difference between the wind and space velocities of the star and makes the contact discontinuity of the bow shock stable for a range of stellar space velocities and mass-loss rates. Our best-fitting model reproduces the overall shape and surface brightness of the observed bow shock and suggests that the space velocity and mass-loss rate of IRC -10414 are ≈50 km s-1 and ≈10-6 M⊙ yr-1, respectively, and that the number density of the local interstellar medium is ≈3 cm-3. It also shows that the bow shock emission comes mainly from the shocked stellar wind. This naturally explains the enhanced nitrogen abundance in the line-emitting material, derived from the spectroscopy of the bow shock. We found that photoionized bow shocks are ≈15-50 times brighter in optical line emission than their neutral counterparts, from which we conclude that the bow shock of IRC -10414 must be photoionized.
Interactions between exoplanets and the winds of young stars
Directory of Open Access Journals (Sweden)
Vidotto A. A.
2014-01-01
Full Text Available The topology of the magnetic field of young stars is important not only for the investigation of magnetospheric accretion, but also responsible in shaping the large-scale structure of stellar winds, which are crucial for regulating the rotation evolution of stars. Because winds of young stars are believed to have enhanced mass-loss rates compared to those of cool, main-sequence stars, the interaction of winds with newborn exoplanets might affect the early evolution of planetary systems. This interaction can also give rise to observational signatures which could be used as a way to detect young planets, while simultaneously probing for the presence of their still elusive magnetic fields. Here, we investigate the interaction between winds of young stars and hypothetical planets. For that, we model the stellar winds by means of 3D numerical magnetohydrodynamic simulations. Although these models adopt simplified topologies of the stellar magnetic field (dipolar fields that are misaligned with the rotation axis of the star, we show that asymmetric field topologies can lead to an enhancement of the stellar wind power, resulting not only in an enhancement of angular momentum losses, but also intensifying and rotationally modulating the wind interactions with exoplanets.
Dissociative Photoionization of Diethyl Ether.
Voronova, Krisztina; Mozaffari Easter, Chrissa M; Covert, Kyle J; Bodi, Andras; Hemberger, Patrick; Sztáray, Bálint
2015-10-29
The dissociative photoionization of internal energy selected diethyl ether ions was investigated by imaging photoelectron photoion coincidence spectroscopy. In a large, 5 eV energy range Et2O(+) cations decay by two parallel and three sequential dissociative photoionization channels, which can be modeled well using statistical theory. The 0 K appearance energies of the CH3CHOCH2CH3(+) (H-loss, m/z = 73) and CH3CH2O═CH2(+) (methyl-loss, m/z = 59) fragment ions were determined to be 10.419 ± 0.015 and 10.484 ± 0.008 eV, respectively. The reemergence of the hydrogen-loss ion above 11 eV is attributed to transition-state (TS) switching, in which the second, outer TS is rate-determining at high internal energies. At 11.81 ± 0.05 eV, a secondary fragment of the CH3CHOCH2CH3(+) (m/z = 73) ion, protonated acetaldehyde, CH3CH═OH(+) (m/z = 45) appears. On the basis of the known thermochemical onset of this fragment, a reverse barrier of 325 meV was found. Two more sequential dissociation reactions were examined, namely, ethylene and formaldehyde losses from the methyl-loss daughter ion. The 0 K appearance energies of 11.85 ± 0.07 and 12.20 ± 0.08 eV, respectively, indicate no reverse barrier in these processes. The statistical model of the dissociative photoionization can also be used to predict the fractional ion abundances in threshold photoionization at large temperatures, which could be of use in, for example, combustion diagnostics.
Theoretical treatment of molecular photoionization based on the R-matrix method
International Nuclear Information System (INIS)
Tashiro, Motomichi
2012-01-01
The R-matrix method was implemented to treat molecular photoionization problem based on the UK R-matrix codes. This method was formulated to treat photoionization process long before, however, its application has been mostly limited to photoionization of atoms. Application of the method to valence photoionization as well as inner-shell photoionization process will be presented.
International Nuclear Information System (INIS)
Browning, G.L.; Holzer, T.E.
1992-01-01
The reduced system of equations commonly used to describe the time evolution of the polar wind and multiconstituent stellar winds is derived from the equations for a multispecies plasma with known temperature profiles by assuming that the electron thermal speed approaches infinity. The reduced system is proved to have unbounded growth near the sonic point of the protons for many of the standard parameter cases. For the same parameter cases, however, the unmodified system (from which the reduced system is derived) exhibits growth in some of the Fourier modes, but this growth is bounded. An alternate system (the approximate system) in which the electron thermal speed is slowed down is introduced. The approximate system retains the mathematical behavior of the unmodified system and can be shown to accurately describe the smooth solutions of the unmodified system. The approximate system has a number of other advantages over the reduced system becomes inaccurate. Also, for three-dimensional flows the correct reduced system requires the solution of an elliptic equation, while the approximate system is hyperbolic and only requires a time step approximately 1 order of magnitude less than the reduced system. Numerical solutions from models based on the two systems are compared with each other to illustrate these points
An alternative approach to condensed-phase photoionization
Energy Technology Data Exchange (ETDEWEB)
Ma Xiaoguang [Department of Physics, Yantai Normal University, Yantai 264025 (China)]. E-mail: hsiaoguangma@163.com
2006-01-02
Starting from Maxwell's equations for the electromagnetic field in a linear Kramers-Kronig dielectric, a general expression for photoionization cross sections of atoms or molecules embedded in a medium and a dielectric influence function (DIF) are derived in this Letter firstly. It is also suggested that a density turning point (DTP) of a photoionization process may be viewed as the critical density N{sub c}({omega}) where the photoionization properties may have notable and different variations with density.
Theoretical Studies on Photoionization Cross Sections of Solid Gold
International Nuclear Information System (INIS)
Ma Xiaoguang; Sun Weiguo; Cheng Yansong
2005-01-01
Accurate expression for photoabsorption (photoionization) cross sections of high density system proposed recently is used to study the photoionization of solid gold. The results show that the present theoretical photoionization cross sections have good agreement both in structure and in magnitude with the experimental results of gold crystal. The studies also indicate that both the real part ε' and the imaginary part ε'' of the complex dielectric constant ε, and the dielectric influence function of a nonideal system have rich structures in low energy side with a range about 50 eV, and suggest that the influence of particle interactions of surrounding particles with the photoionized particle on the photoionization cross sections can be easily investigated using the dielectric influence function. The electron overlap effects are suggested to be implemented in the future studies to improve the accuracy of theoretical photoionization cross sections of a solid system.
International Nuclear Information System (INIS)
Van Buren, D.
1985-01-01
Using the Michigan HD catalog volumes I--III, the all-sky sample of O stars of Garmany, Conti, and Chiosi, Lucke's map of the distribution of obscuring material within 2 kpc, and an amalgam of recent stellar evolution calculations, the number of stars formed kpc -2 yr -1 [log (M/M/sub sun/)] -1 (IMF) is psi = 5.4 x 10 -4 (M/M/sub sun/)/sup -1.03/. A calibration of mass-loss rates with stellar parameters based on published data yields m = 2.0 x 10 -13 (L/L/sub sun/)/sup 1.25/M/sub sun/ yr -1 . Energy injection into the ISM by winds and supernovae balances mechanical energy dissipation via cloud-cloud collisions. For stars M>5 M/sub sun/ there is near balance between the rate at which mass is turned into stars and the rate at which it is lost from them, implying small remnant masses
Molecular photoionization dynamics
International Nuclear Information System (INIS)
Dehmer, J.L.
1982-01-01
This program seeks to develop both physical insight and quantitative characterization of molecular photoionization processes. Progress is briefly described, and some publications resulting from the research are listed
Photoionization of Ar2 at high resolution
International Nuclear Information System (INIS)
Dehmer, P.M.
1982-01-01
The relative photoionization cross section of Ar 2 was determined at a resolution of 0.07 A in the wavelength region from 800 to 850 A using a new photoionization mass spectrometer that combines a high intensity helium continuum lamp with a free supersonic molecular beam source. In the region studied, the photoionization cross section is dominated by autoionization of molecular Rydberg states, and the structure is diffuse owing to the combined effects of autoionization and predissociation. The molecular photoionization spectrum is extremely complex and shows little resemblence either to the corresponding atomic spectrum (indicating that the spectrum of the dimer is not simply a perturbed atomic spectrum) or to the molecular absorption spectrum at longer wavelengths. The regular vibrational progressions seen at longer wavelengths are absent above the first ionization potential. Detailed spectroscopic analysis is possible for only a small fraction of the observed features; however, vibrational intervals of 50--100 cm -1 suggest that some of the Rydberg states have B 2 Pi/sub 3/2g/ ionic cores. A comparison of the absorption and photoionization spectra shows that, at wavelengths shorter than approx.835 A, many of the excited states decay via mechanisms other than autoionization
Theory of attosecond delays in molecular photoionization.
Baykusheva, Denitsa; Wörner, Hans Jakob
2017-03-28
We present a theoretical formalism for the calculation of attosecond delays in molecular photoionization. It is shown how delays relevant to one-photon-ionization, also known as Eisenbud-Wigner-Smith delays, can be obtained from the complex dipole matrix elements provided by molecular quantum scattering theory. These results are used to derive formulae for the delays measured by two-photon attosecond interferometry based on an attosecond pulse train and a dressing femtosecond infrared pulse. These effective delays are first expressed in the molecular frame where maximal information about the molecular photoionization dynamics is available. The effects of averaging over the emission direction of the electron and the molecular orientation are introduced analytically. We illustrate this general formalism for the case of two polyatomic molecules. N 2 O serves as an example of a polar linear molecule characterized by complex photoionization dynamics resulting from the presence of molecular shape resonances. H 2 O illustrates the case of a non-linear molecule with comparably simple photoionization dynamics resulting from a flat continuum. Our theory establishes the foundation for interpreting measurements of the photoionization dynamics of all molecules by attosecond metrology.
Weaving the history of the solar wind with magnetic field lines
Alvarado Gomez, Julian
2017-08-01
Despite its fundamental role for the evolution of the solar system, our observational knowledge of the wind properties of the young Sun comes from a single stellar observation. This unexpected fact for a field such as astrophysics arises from the difficulty of detecting Sun-like stellar winds. Their detection relies on the appearance of an astrospheric signature (from the stellar wind-ISM interaction region), visible only with the aid of high-resolution HST Lyman-alpha spectra. However, observations and modelling of the present day Sun have revealed that magnetic fields constitute the main driver of the solar wind, providing guidance on how such winds would look like back in time. In this context we propose observations of four young Sun-like stars in order to detect their astrospheres and characterise their stellar winds. For all these objects we have recovered surface magnetic field maps using the technique of Zeeman Doppler Imaging, and developed detailed wind models based on these observed field distributions. Even a single detection would represent a major step forward for our understanding of the history of the solar wind, and the outflows in more active stars. Mass loss rate estimates from HST will be confronted with predictions from realistic models of the corona/stellar wind. In one of our objects the comparison would allow us to quantify the wind variability induced by the magnetic cycle of a star, other than the Sun, for the first time. Three of our targets are planet hosts, thus the HST spectra would also provide key information on the high-energy environment of these systems, guaranteeing their legacy value for the growing field of exoplanet characterisation.
AN EXPLORATION OF THE STATISTICAL SIGNATURES OF STELLAR FEEDBACK
Energy Technology Data Exchange (ETDEWEB)
Boyden, Ryan D.; Offner, Stella S. R. [Department of Astronomy, University of Massachusetts, Amherst, MA 01003 (United States); Koch, Eric W.; Rosolowsky, Erik W., E-mail: soffner@astro.umass.edu [Department of Physics, University of Alberta, Edmonton, T6G 2E1 (Canada)
2016-12-20
All molecular clouds are observed to be turbulent, but the origin, means of sustenance, and evolution of the turbulence remain debated. One possibility is that stellar feedback injects enough energy into the cloud to drive observed motions on parsec scales. Recent numerical studies of molecular clouds have found that feedback from stars, such as protostellar outflows and winds, injects energy and impacts turbulence. We expand upon these studies by analyzing magnetohydrodynamic simulations of molecular clouds, including stellar winds, with a range of stellar mass-loss rates and magnetic field strengths. We generate synthetic {sup 12}CO(1–0) maps assuming that the simulations are at the distance of the nearby Perseus molecular cloud. By comparing the outputs from different initial conditions and evolutionary times, we identify differences in the synthetic observations and characterize these using common astrostatistics. We quantify the different statistical responses using a variety of metrics proposed in the literature. We find that multiple astrostatistics, including the principal component analysis, the spectral correlation function, and the velocity coordinate spectrum (VCS), are sensitive to changes in stellar mass-loss rates and/or time evolution. A few statistics, including the Cramer statistic and VCS, are sensitive to the magnetic field strength. These findings demonstrate that stellar feedback influences molecular cloud turbulence and can be identified and quantified observationally using such statistics.
Application of the R-matrix method to photoionization of molecules.
Tashiro, Motomichi
2010-04-07
The R-matrix method has been used for theoretical calculation of electron collision with atoms and molecules for long years. The method was also formulated to treat photoionization process, however, its application has been mostly limited to photoionization of atoms. In this work, we implement the R-matrix method to treat molecular photoionization problem based on the UK R-matrix codes. This method can be used for diatomic as well as polyatomic molecules, with multiconfigurational description for electronic states of both target neutral molecule and product molecular ion. Test calculations were performed for valence electron photoionization of nitrogen (N(2)) as well as nitric oxide (NO) molecules. Calculated photoionization cross sections and asymmetry parameters agree reasonably well with the available experimental results, suggesting usefulness of the method for molecular photoionization.
Double Photoionization Near Threshold
Wehlitz, Ralf
2007-01-01
The threshold region of the double-photoionization cross section is of particular interest because both ejected electrons move slowly in the Coulomb field of the residual ion. Near threshold both electrons have time to interact with each other and with the residual ion. Also, different theoretical models compete to describe the double-photoionization cross section in the threshold region. We have investigated that cross section for lithium and beryllium and have analyzed our data with respect to the latest results in the Coulomb-dipole theory. We find that our data support the idea of a Coulomb-dipole interaction.
Inner-shell photoionization in weak and strong radiation fields
International Nuclear Information System (INIS)
Southworth, S.H.; Dunford, R.W.; Ederer, D.L.; Kanter, E.P.; Kraessig, B.; Young, L.
2004-01-01
The X-ray beams presently produced at synchrotron-radiation facilities interact weakly with matter, and the observation of double photoionization is due to electron-electron interactions. The intensities of future X-ray free-electron lasers are expected to produce double photoionization by absorption of two photons. The example of double K-shell photoionization of neon is discussed in the one- and two-photon cases. We also describe an experiment in which X rays photoionize the K shell of krypton in the presence of a strong AC field imposed by an optical laser
Spectra of resonance surface photoionization
Energy Technology Data Exchange (ETDEWEB)
Antsiferov, V.V.; Smirnov, G.I.; Telegin, G.G. [Budker Nuclear Physics Institute, Novosibirsk (Russian Federation)
1995-09-01
The theory of nonactivated electron transfer between atoms interacting reasonantly with coherent radiation and a metal surface is developed. The spectral resonances in photoabsorption and surface photoionization are found to be related to nonlinear interference effects in the interaction between discrete atomic levels and the continuum formed by the quasi-continuous electron spectrum of a normal metal. The asymmetry in the resonance surface photoionization spectrum is shown to have a shape typical of the Fano autoionization resonances. 18 refs.
Design, construction and validation of the UST-1 modular stellarator
Energy Technology Data Exchange (ETDEWEB)
Queral, V., E-mail: vicentemanuel.queral@ciemat.es
2016-11-15
Highlights: • A small and simple low cost two period modular stellarator is reviewed. • It is defined as a monolithic circular surface torus with carved grooves. • The grooves are accurately mechanised by a new toroidal milling machine. • A very simple e-beam field mapping system has been built and utilized. - Abstract: Stellarator advancement is hindered, among others, by the requirement of geometric complexity at high accuracy and the still scarce universities and research centres following the stellarator line. In this framework, the objectives of the small UST-1 stellarator development were to: (i) explore and test the performance of one possible accurate construction method for stellarators (ii) encourage universities and small fusion research centres to build simple and economical stellarators (iii) educative purpose. Therefore, UST-1 was properly designed to be easily built by a milling machine working on toroidal coordinates, being the winding surface circular poloidally and toroidally. The coil frame is a sole monolithic toroidal thick surface equipped with grooves mechanised by the toroidal milling machine. Only one double pancake is wound in each groove so as to compress the conductor on the laterals of the groove in order to speed up and simplify the winding process. The physics design, the conceptual engineering design and the construction process of UST-1 is presented. The toroidal milling machine is described. The e-beam field line mapping experiments carried out to validate the resulting magnetic configuration are reported. The developed construction method has been proved for the small UST-1 stellarator. Small stellarators are valuable for quick tests of diagnostics, educative purposes, assessment of new confinement concepts, turbulence studies and other applications.
Design, construction and validation of the UST-1 modular stellarator
International Nuclear Information System (INIS)
Queral, V.
2016-01-01
Highlights: • A small and simple low cost two period modular stellarator is reviewed. • It is defined as a monolithic circular surface torus with carved grooves. • The grooves are accurately mechanised by a new toroidal milling machine. • A very simple e-beam field mapping system has been built and utilized. - Abstract: Stellarator advancement is hindered, among others, by the requirement of geometric complexity at high accuracy and the still scarce universities and research centres following the stellarator line. In this framework, the objectives of the small UST-1 stellarator development were to: (i) explore and test the performance of one possible accurate construction method for stellarators (ii) encourage universities and small fusion research centres to build simple and economical stellarators (iii) educative purpose. Therefore, UST-1 was properly designed to be easily built by a milling machine working on toroidal coordinates, being the winding surface circular poloidally and toroidally. The coil frame is a sole monolithic toroidal thick surface equipped with grooves mechanised by the toroidal milling machine. Only one double pancake is wound in each groove so as to compress the conductor on the laterals of the groove in order to speed up and simplify the winding process. The physics design, the conceptual engineering design and the construction process of UST-1 is presented. The toroidal milling machine is described. The e-beam field line mapping experiments carried out to validate the resulting magnetic configuration are reported. The developed construction method has been proved for the small UST-1 stellarator. Small stellarators are valuable for quick tests of diagnostics, educative purposes, assessment of new confinement concepts, turbulence studies and other applications.
Inner-shell photoionization of group-IIB atoms
International Nuclear Information System (INIS)
Kutzner, M.; Tidwell, C.; Vance, S.E.; Radojevic, V.
1994-01-01
Total and partial photoionization cross sections, branching ratios, and angular-distribution asymmetry parameters for inner subshells (nl,l≥2) of the group-IIB elements zinc, cadmium, and mercury have been calculated in both the relativistic random-phase approximation and the relativistic random-phase approximation modified to include relaxation. Comparisons are made between the results of the two theoretical methods and with experiment where available. The present theoretical results for the 3d inner-shell photoionization of zinc are not in accord with experiment. We confirm previous work [S. L. Carter and H. P. Kelly, J. Phys. B 11, 2467 (1978)] which demonstrated that relaxation is an important effect in photoionization of the 4d subshell of atomic cadmium. It is also found that the inclusion of relaxation effects resolves a discrepancy between theory and experiment for the 4f inner-shell photoionization of atomic mercury
ON THE MAXIMUM MASS OF STELLAR BLACK HOLES
International Nuclear Information System (INIS)
Belczynski, Krzysztof; Fryer, Chris L.; Bulik, Tomasz; Ruiter, Ashley; Valsecchi, Francesca; Vink, Jorick S.; Hurley, Jarrod R.
2010-01-01
We present the spectrum of compact object masses: neutron stars and black holes (BHs) that originate from single stars in different environments. In particular, we calculate the dependence of maximum BH mass on metallicity and on some specific wind mass loss rates (e.g., Hurley et al. and Vink et al.). Our calculations show that the highest mass BHs observed in the Galaxy M bh ∼ 15 M sun in the high metallicity environment (Z = Z sun = 0.02) can be explained with stellar models and the wind mass loss rates adopted here. To reach this result we had to set luminous blue variable mass loss rates at the level of ∼10 -4 M sun yr -1 and to employ metallicity-dependent Wolf-Rayet winds. With such winds, calibrated on Galactic BH mass measurements, the maximum BH mass obtained for moderate metallicity (Z = 0.3 Z sun = 0.006) is M bh,max = 30 M sun . This is a rather striking finding as the mass of the most massive known stellar BH is M bh = 23-34 M sun and, in fact, it is located in a small star-forming galaxy with moderate metallicity. We find that in the very low (globular cluster-like) metallicity environment the maximum BH mass can be as high as M bh,max = 80 M sun (Z = 0.01 Z sun = 0.0002). It is interesting to note that X-ray luminosity from Eddington-limited accretion onto an 80 M sun BH is of the order of ∼10 40 erg s -1 and is comparable to luminosities of some known ultra-luminous X-ray sources. We emphasize that our results were obtained for single stars only and that binary interactions may alter these maximum BH masses (e.g., accretion from a close companion). This is strictly a proof-of-principle study which demonstrates that stellar models can naturally explain even the most massive known stellar BHs.
Photoionization by a bichromatic field: Adiabatic theory
International Nuclear Information System (INIS)
Pazdzersky, V.A.; Yurovsky, V.A.
1995-01-01
Atom photoionization by the superposition of a fundamental field and its second harmonic is considered. The finite analytical expressions for the photoionization probability are obtained using the adiabatic approximation. They demonstrate that the photoelectron angular distribution has a polar symmetry when the electrical field strength has a maximal polar asymmetry and the distribution is asymmetrical when the field is symmetrical. A strict proof of the polar symmetry of the photoionization probability in the case of the electrical field with maximal asymmetry is deduced using the Keldysh-Faisal-Reiss theories. The obtained results are in agreement with the experimental data available
Stellarmak a hybrid stellarator: Spheromak
International Nuclear Information System (INIS)
Hartman, C.W.
1980-01-01
This paper discusses hybridization of modified Stellarator-like transform windings (T-windings) with a Spheromak or Field-Reversed-Mirror configuration. This configuration, Stellarmak, retains the important topological advantage of the Spheromak or FRM of having no plasma linking conductors or blankets. The T-windings provide rotational transformation in toroidal angle of the outer poloidal field lines, in effect creating a reversed B/sub Toroidal/ Spheromak or adding average B/sub T/ to the FRM producing higher shear, increased limiting β, and possibly greater stability to kinks and tilt. The presence of field ripple in the toroidal direction may be sufficient to inhibit cancellation of directed ion current by electron drag to allow steady state operation with the toroidal as well as poloidal current maintained by neutral beams
Nonthermal and screening effects on photoionizations in Lorentzian plasmas
International Nuclear Information System (INIS)
Shin, Dong-Soo; Jung, Young-Dae
2009-01-01
The nonthermal and plasma screening effects on the x-ray photoionization process are investigated in astrophysical Lorentzian plasmas. The screened atomic wave function and energy eigenvalue of the target ion in Lorentzian plasmas are obtained by the Rayleigh-Ritz variational method. The x-ray retardation and screened Coulomb corrections are considered to obtain a photoionization cross section as a function of the spectral index and plasma parameters. It is shown that the nonthermal character of the Lorentzian plasma suppresses the photoionization cross section. Hence, the photoionization cross sections in nonthermal plasmas are found to be always smaller than those in thermal plasmas. It is also shown that the plasma screening effect is more significant for small spectral indices. In addition, the nonthermal effect on the photoionization cross section is found to be decreased with an increase in the Debye length.
Attosecond Delays in Molecular Photoionization.
Huppert, Martin; Jordan, Inga; Baykusheva, Denitsa; von Conta, Aaron; Wörner, Hans Jakob
2016-08-26
We report measurements of energy-dependent photoionization delays between the two outermost valence shells of N_{2}O and H_{2}O. The combination of single-shot signal referencing with the use of different metal foils to filter the attosecond pulse train enables us to extract delays from congested spectra. Remarkably large delays up to 160 as are observed in N_{2}O, whereas the delays in H_{2}O are all smaller than 50 as in the photon-energy range of 20-40 eV. These results are interpreted by developing a theory of molecular photoionization delays. The long delays measured in N_{2}O are shown to reflect the population of molecular shape resonances that trap the photoelectron for a duration of up to ∼110 as. The unstructured continua of H_{2}O result in much smaller delays at the same photon energies. Our experimental and theoretical methods make the study of molecular attosecond photoionization dynamics accessible.
A Wolf-Rayet-Like Progenitor of SN 2013cu from Spectral Observations of a Stellar Wind
Gal-Yam, Avishay; Arcavi, I.; Ofek, E. O.; Ben-Ami, S.; Cenko, S. B.; Kasliwal, M. M.; Cao, Y.; Yaron, O.; Tal, D.; Silverman, J. M.;
2014-01-01
The explosive fate of massive Wolf-Rayet stars (WRSs) is a key open question in stellar physics. An appealing option is that hydrogen- deficient WRSs are the progenitors of some hydrogen-poor supernova explosions of types IIb, Ib and Ic. A blue object, having luminosity and colours consistent with those of some WRSs, has recently been identified in pre-explosion images at the location of a supernova of type Ib, but has not yet been conclusively determined to have been the progenitor. Similar work has so far only resulted in non-detections. Comparison of early photometric observations of type Ic supernovae with theoretical models suggests that the progenitor stars had radii of less than 10(exp 12) centimetres, as expected for some WRSs. The signature of WRSs, their emission line spectra, cannot be probed by such studies. Here we report the detection of strong emission lines in a spectrum of type IIb supernova 2013cu (iPTF13ast) obtained approximately 15.5 hours after explosion (by 'flash spectroscopy', which captures the effects of the supernova explosion shock breakout flash on material surrounding the progenitor star).We identify Wolf-Rayet-like wind signatures, suggesting a progenitor of the WN(h) subclass (those WRSs with winds dominated by helium and nitrogen, with traces of hydrogen). The extent of this dense wind may indicate increased mass loss from the progenitor shortly before its explosion, consistent with recent theoretical predictions.
Dissociative Photoionization of the Elusive Vinoxy Radical.
Adams, Jonathan D; Scrape, Preston G; Lee, Shih-Huang; Butler, Laurie J
2017-08-24
These experiments report the dissociative photoionization of vinoxy radicals to m/z = 15 and 29. In a crossed laser-molecular beam scattering apparatus, we induce C-Cl bond fission in 2-chloroacetaldehyde by photoexcitation at 157 nm. Our velocity measurements, combined with conservation of angular momentum, show that 21% of the C-Cl photofission events form vinoxy radicals that are stable to subsequent dissociation to CH 3 + CO or H + ketene. Photoionization of these stable vinoxy radicals, identified by their velocities, which are momentum-matched with the higher-kinetic-energy Cl atom photofragments, shows that the vinoxy radicals dissociatively photoionize to give signal at m/z = 15 and 29. We calibrated the partial photoionization cross section of vinoxy to CH 3 + relative to the bandwidth-averaged photoionization cross section of the Cl atom at 13.68 eV to put the partial photoionization cross sections on an absolute scale. The resulting bandwidth-averaged partial cross sections are 0.63 and 1.3 Mb at 10.5 and 11.44 eV, respectively. These values are consistent with the upper limit to the cross section estimated from a study by Savee et al. on the O( 3 P) + propene bimolecular reaction. We note that the uncertainty in these values is primarily dependent on the signal attributed to C-Cl primary photofission in the m/z = 35 (Cl + ) time-of-flight data. While the value is a rough estimate, the bandwidth-averaged partial photoionization cross section of vinoxy to HCO + calculated from the signal at m/z = 29 at 11.53 eV is approximately half that of vinoxy to CH 3 + . We also present critical points on the potential energy surface of the vinoxy cation calculated at the G4//B3LYP/6-311++G(3df,2p) level of theory to support the observation of dissociative ionization of vinoxy to both CH 3 + and HCO + .
Relativistic Photoionization Computations with the Time Dependent Dirac Equation
2016-10-12
Naval Research Laboratory Washington, DC 20375-5320 NRL/MR/6795--16-9698 Relativistic Photoionization Computations with the Time Dependent Dirac... Photoionization Computations with the Time Dependent Dirac Equation Daniel F. Gordon and Bahman Hafizi Naval Research Laboratory 4555 Overlook Avenue, SW...Unclassified Unlimited Unclassified Unlimited 22 Daniel Gordon (202) 767-5036 Tunneling Photoionization Ionization of inner shell electrons by laser
Component Manufacturing Development for the National Compact Stellarator Experiment (NCSX)
International Nuclear Information System (INIS)
Heitzenroeder, P.J.; Brown, T.G.; Chrzanowski, J.H.; Cole, M.J.; Goranson, P.L.; Neilson, G.H.; Nelson, B.E.; Reiersen, W.T.; Sutton, L.L.; Williamson, D.E.; Viola, M.E.
2004-11-01
NCSX [National Compact Stellarator Experiment] is the first of a new class of stellarators called compact stellarators which hold the promise of retaining the steady state feature of the stellarator but at a much lower aspect ratio and using a quasi-axisymmetric magnetic field to obtain tokamak-like performance. Although much of NCSX is conventional in design and construction, the vacuum vessel and modular coils provide significant engineering challenges due to their complex shapes, need for high dimensional accuracy, and the high current density required in the modular coils due space constraints. Consequently, a three-phase development program has been undertaken. In the first phase, laboratory/industrial studies were performed during the development of the conceptual design to permit advances in manufacturing technology to be incorporated into NCSX's plans. In the second phase, full-scale prototype modular coil winding forms, compacted cable conductors, and 20 degree sectors of the vacuum vessel were fabricated in industry. In parallel, the NCSX project team undertook RandD studies that focused on the windings. The third (production) phase began in September 2004. First plasma is scheduled for January 2008
A DETECTION OF GAS ASSOCIATED WITH THE M31 STELLAR STREAM
Energy Technology Data Exchange (ETDEWEB)
Koch, Andreas [Zentrum für Astronomie der Universität Heidelberg, Landessternwarte, Königstuhl 12, D-69117 Heidelberg (Germany); Danforth, Charles W.; Keeney, Brian A. [CASA, Department of Astrophysical and Planetary Sciences, University of Colorado, 389-UCB, Boulder, CO 80309 (United States); Rich, R. Michael [Physics and Astronomy Building, 430 Portola Plaza, Box 951547, Department of Physics and Astronomy, University of California, Los Angeles, CA 90095 (United States); Ibata, Rodrigo [Observatoire de Strasbourg, 11, rue de l’Université, F-67000, Strasbourg (France)
2015-07-10
Detailed studies of stellar populations in the halos of the Milky Way and the Andromeda (M31) galaxies have shown increasing numbers of tidal streams and dwarf galaxies, attesting to a complicated and on-going process of hierarchical structure formation. The most prominent feature in the halo of M31 is the Giant Stellar Stream, a structure ∼4.°5 in extent along the sky, which is close to, but not coincident with the galaxy's minor axis. The stars that make up this stream are kinematically and chemically distinct from the other stars in the halo. Here, we present Hubble Space Telescope/Cosmic Origins Spectrograph high-resolution ultraviolet absorption spectra of three active galactic nuclei sight lines which probe the M31 halo, including one that samples gas in the main southwestern portion of the Giant Stream. We see two clear absorption components in many metal species at velocities typical of the M31 halo and a third, blueshifted component which arises in the stream. Photoionization modeling of the column density ratios in the different components shows gas in an ionization state typical of that seen in other galaxy halo environments and suggests solar to slightly super-solar metallicity, consistent with previous findings from stellar spectroscopy.
EXCLUSION OF COSMIC RAYS IN PROTOPLANETARY DISKS: STELLAR AND MAGNETIC EFFECTS
International Nuclear Information System (INIS)
Cleeves, L. Ilsedore; Adams, Fred C.; Bergin, Edwin A.
2013-01-01
Cosmic rays (CRs) are thought to provide an important source of ionization in the outermost and densest regions of protoplanetary disks; however, it is unknown to what degree they are physically present. As is observed in the solar system, stellar winds can inhibit the propagation of CRs within the circumstellar environment and subsequently into the disk. In this work, we explore the hitherto neglected effects of CR modulation by both stellar winds and magnetic field structures and study how these processes act to reduce disk ionization rates. We construct a two-dimensional protoplanetary disk model of a T-Tauri star system, focusing on ionization from stellar and interstellar FUV, stellar X-ray photons, and CRs. We show that stellar winds can power a heliosphere-like analog, i.e., a ''T-Tauriosphere,'' diminishing CR ionization rates by several orders of magnitude at low to moderate CR energies (E CR ≤ 1 GeV). We explore models of both the observed solar wind CR modulation and a highly simplified estimate for ''elevated'' CR modulation as would be expected from a young T-Tauri star. In the former (solar analog) case, we estimate the ionization rate from galactic CRs to be ζ CR ∼ (0.23-1.4) × 10 –18 s –1 . This range of values, which we consider to be the maximum CR ionization rate for the disk, is more than an order of magnitude lower than what is generally assumed in current models for disk chemistry and physics. In the latter elevated case, i.e., for a ''T-Tauriosphere,'' the ionization rate by CRs is ζ CR ∼ –20 s –1 , which is 1000 times smaller than the interstellar value. We discuss the implications of a diminished CR ionization rate on the gas physics by estimating the size of the resulting magnetorotational instability dead zones. Indeed, if winds are as efficient at CR modulation as predicted here, short-lived radionuclides (now extinct) would have provided the major source of ionization (ζ RN ∼ 7.3 × 10 –19 s –1 ) in the planet
Attosecond interference control of XUV photoionization
Energy Technology Data Exchange (ETDEWEB)
Cao Wei; Lu Peixiang; Lan Pengfei; Li Yuhua; Wang Xinlin [Wuhan National Laboratory for Optoelectronics and School of Optoelectronics Science and Engineering, Huazhong University of Science and Technology, Wuhan 430074 (China)], E-mail: lupeixiang@mail.hust.edu.cn
2008-04-28
The characterizing of attosecond pulses has great importance for the investigation of ultrafast phenomena. Here, we proposed a novel and efficient scheme for measuring attosecond XUV pulses, which is based on laser-dressed XUV photoionization. The ultrashort attosecond gating of photoionization leads to an interference structure in the photoelectron spectrum. Then the duration of the attosecond XUV pulse can be retrieved directly from the photoelectron spectrum with a rather high resolution.
Attosecond interference control of XUV photoionization
International Nuclear Information System (INIS)
Cao Wei; Lu Peixiang; Lan Pengfei; Li Yuhua; Wang Xinlin
2008-01-01
The characterizing of attosecond pulses has great importance for the investigation of ultrafast phenomena. Here, we proposed a novel and efficient scheme for measuring attosecond XUV pulses, which is based on laser-dressed XUV photoionization. The ultrashort attosecond gating of photoionization leads to an interference structure in the photoelectron spectrum. Then the duration of the attosecond XUV pulse can be retrieved directly from the photoelectron spectrum with a rather high resolution
Photoionization and cold collision studies using trapped atoms
International Nuclear Information System (INIS)
Gould, P.L.
1996-01-01
The authors have used laser cooling and trapping techniques to investigate photoionization and cold collisions. With laser-trapped Rb, they have measured the photoionization cross section from the first excited (5P) level by observing the photoionization-induced loss rate of neutral atoms from the trap. This technique has the advantage that it directly measures the photoionization rate per atom. Knowing the ionizing laser intensity and the excited-state fraction, the measured loss rate gives the absolute cross section. Using this technique, the Rb 5P photoionization cross section at ∼400 nm has been determined with an uncertainty of 9%. The authors are currently attempting to extend this method to the 5D level. Using time-ordered pulses of diode-laser light (similar to the STIRAP technique), they have performed very efficient two-photon excitation of trapped Rb atoms to 5D. Finally, they will present results from a recent collaboration which combines measurements form conventional molecular spectroscopy (single photon and double resonance) with photoassociation collisions of ultracold Na atoms to yield a precise (≤1 ppm) value for the dissociation energy of the X Σ g+ ground state of the Na 2 molecule
EMISSION SPECTRUM OF HELIUM-LIKE IONS IN PHOTOIONIZED PLASMAS
International Nuclear Information System (INIS)
Wang, Feilu; Salzmann, David; Zhao, Gang; Takabe, Hideaki
2012-01-01
The aim of the present paper is to investigate the influence of inner-shell photoionization and photoexcitation on He α and its satellite's spectra in photoionized plasmas. An analysis is carried out on the relative importance of the various atomic processes in photoionized plasmas as a function of the electron temperature and irradiation conditions. In particular, we investigate the influence of K-shell photoionization of Li-like ions on the He α spectrum and of Be-like ions on the He α satellites. It is found that in photoionized plasmas these inner-shell processes contribute significantly under low radiation temperature and/or intensity, when Li- and Be-like ions are highly abundant but highly ionized H-like ions are rare. A short discussion is presented about the parameter space in which the excited 1s2p state has statistical or non-statistical distributions, and how such distributions affect the emission spectrum.
Photoionization of Li and Na in Debye plasma environments
International Nuclear Information System (INIS)
Sahoo, Satyabrata; Ho, Y.K.
2006-01-01
A calculation of the photoionization cross sections is presented for alkali-metal atoms such as Li and Na in plasma environments. The computational scheme is based on the complex coordinate rotation method. A model potential formalism has been used to simplify the computational complexity of the problems of making quantitative predictions of properties and interactions of many electron systems in Debye plasmas. The plasma environment is found to appreciably influence the photoionization cross sections. In this regard the photoionization cross sections of isolated atoms are also discussed that is found to be in good agreement with the previous theoretical results. It is observed that the strong plasma screening effect remarkably alters the photoionization cross sections near the ionization threshold. The Cooper minimum in the photoionization cross sections of Na shifts toward the higher energy as the plasma screening effect increases. For Li, the Cooper minimum is uncovered in strong plasma environments. This is the first time such structures have been determined
Theoretical Studies on Expressions of Condensed-Phase Photoionization Cross Section
International Nuclear Information System (INIS)
Ma Xiaoguang; Wang Meishan; Wang Dehua; Qu Zhaojun
2006-01-01
A set of general expressions for photoionization cross sections of atoms or molecules embedded in a medium and a dielectric influence function are derived based on Maxwell's equations and the Beer-Lambert's law in this work. The applications are performed for the photoionization process of solid gold both in the Clausius-Mossotti (virtual cavity) model and the Glauber-Lewenstein (real cavity) model firstly. The results show that the present theoretical expressions of photoionization cross section can be used to describe the photoionization process of atoms in condensed matter properly.
K-shell photoionizations in classical nonideal plasmas
International Nuclear Information System (INIS)
Jung, Young-Dae
2001-01-01
Collective and plasma screening effects on photoionization cross sections from the 1s state of hydrogenic ions in classical nonideal plasmas are investigated. An effective pseudopotential model taking into account the collective and plasma screening effects is applied to describe the interaction potential in nonideal plasmas. The screened atomic wave function and energy eigenvalue for the ground state of the hydrogenic ion in classical nonideal plasmas are obtained by the Ritz variational method. The photoionization cross section is obtained by the acceleration form of the transition matrix element in order to investigate the collective and plasma screening effects on the interaction potential. The retardation and Coulomb correction effects are also considered in nonideal plasmas. The total correlation effect is obtained as a function of the nonideality plasma parameter, Debye length, and incident photon energy. The result shows that the collective effect significantly reduces the photoionization cross section. It is also found that the collective effect on the photoionization cross section is increased with increasing the incident photon energy
Photoionization-photoelectron research
Energy Technology Data Exchange (ETDEWEB)
Berkowitz, J.; Ruscic, B. [Argonne National Laboratory, IL (United States)
1993-12-01
The photoionization research program is aimed at understanding the basic processes of interaction of vacuum ultraviolet (VUV) light with atoms and molecules. This research provides valuable information on both thermochemistry and dynamics. Recent studies include atoms, clusters, hydrides, sulfides and an important fluoride.
Magnetohydrodynamic theory of plasma equilibrium and stability in stellarators: Survey of results
International Nuclear Information System (INIS)
Shafranov, V.D.
1983-01-01
The main advantage of a stellarator is its capability of steady-state operation. It can be exploited as a reactor if stable plasma confinement can be achieved with #betta#approx.10%. Therefore, this limiting pressure value is a key factor in stellarator development. This paper contains a survey of current ideas on the magnetohydrodynamic equilibrium and stability properties of stellarators with sufficiently high pressure. Here, any system of nested toroidal magnetic surfaces generated by external currents is considered a stellarator. Systems produced by helical or equivalent windings, including torsatrons and heliotrons, will be called ordinary stellarators, in contrast to those with spatial axes. It is shown that adequate confinement can be achieved
Thermal radio emission from the winds of single stars
International Nuclear Information System (INIS)
Abbott, D.C.
1985-01-01
Observations of thermal emission at radio wavelengths provides a powerful diagnostic of the rate of mass loss and temperature of the winds of early-type stars. Some winds are also strong sources of nonthermal emission. Case studies of known thermal and nonthermal sources provide empirical criteria for classifying the observed radio radiation. Mass loss rates are derived for 37 OB and Wolf-Rayet stars considered definite or probable thermal wind sources by these criteria. The rate of mass loss is strongly linked to stellar luminosity in OB stars and probably linked to stellar mass in Wolf-Rayet stars, with no measurable correlation with any other stellar property. A few late-type giants and supergiants also have detectable thermal emission, which arises from extended, accelerating, partially-ionized chromospheres. (orig.)
Gas expulsion vs gas retention in young stellar clusters II: effects of cooling and mass segregation
Silich, Sergiy; Tenorio-Tagle, Guillermo
2018-05-01
Gas expulsion or gas retention is a central issue in most of the models for multiple stellar populations and light element anti-correlations in globular clusters. The success of the residual matter expulsion or its retention within young stellar clusters has also a fundamental importance in order to understand how star formation proceeds in present-day and ancient star-forming galaxies and if proto-globular clusters with multiple stellar populations are formed in the present epoch. It is usually suggested that either the residual gas is rapidly ejected from star-forming clouds by stellar winds and supernova explosions, or that the enrichment of the residual gas and the formation of the second stellar generation occur so rapidly, that the negative stellar feedback is not significant. Here we continue our study of the early development of star clusters in the extreme environments and discuss the restrictions that strong radiative cooling and stellar mass segregation provide on the gas expulsion from dense star-forming clouds. A large range of physical initial conditions in star-forming clouds which include the star-forming cloud mass, compactness, gas metallicity, star formation efficiency and effects of massive stars segregation are discussed. It is shown that in sufficiently massive and compact clusters hot shocked winds around individual massive stars may cool before merging with their neighbors. This dramatically reduces the negative stellar feedback, prevents the development of the global star cluster wind and expulsion of the residual and the processed matter into the ambient interstellar medium. The critical lines which separate the gas expulsion and the gas retention regimes are obtained.
Photoionization cross section of atomic and molecular oxygen
International Nuclear Information System (INIS)
Pareek, P.N.
1983-01-01
Photoionization cross sections of atomic oxygen and dissociative photoionization cross sections of molecular oxygen were measured from their respective thresholds to 120 angstrom by use of a photoionization mass spectrometer in conjunction with a spark light source. The photoionization cross sections O 2 + parent ion and O + fragment ion from neutral O 2 were obtained by a technique that eliminated the serious problem of identifying the true abundances of O + ions. These ions are generally formed with considerable kinetic energy and, because most mass spectrometers discriminate against energetic ions, true O + abundances are difficult to obtain. In the present work the relative cross sections for producing O + ions are obtained and normalized against the total cross sections in a spectral region where dissociative ionization is not possible. The fragmentation cross sections for O + were then obtained by subtraction of O 2 + cross sections from the known total photoionization cross sections. The results are compared with the previously published measurements. The absolute photoionization cross section of atomic oxygen sigma 8 /sub +/ was measured at 304 A. The actual number density of oxygen atoms within the ionization region was obtained by measuring the fraction of 0 2 molecules dissociated. This sigma/sub +/ at 304 angstrom was used to convert the relative photoinization cross sections, measured as a function of wavelength using a calibrated photodiode, to absolute cross sections. The results are compared with previous measurements and calculated cross sections. angstrom Rydberg series converging to the OII 4 P state was observed
THE OPTICAL STRUCTURE OF THE STARBURST GALAXY M82. I. DYNAMICS OF THE DISK AND INNER-WIND
International Nuclear Information System (INIS)
Westmoquette, M. S.; Smith, L. J.; Konstantopoulos, I. S.; Gallagher, J. S.; Trancho, G.; Bastian, N.
2009-01-01
We present Gemini-North GMOS-IFU observations of the central starburst clumps and inner wind of M82, together with WIYN DensePak IFU observations of the inner 2 x 0.9 kpc of the disk. These cover the emission lines of Hα, [N II], [S II], and [S III] at a spectral resolution of 45-80 km s -1 . The high signal-to-noise of the data is sufficient to accurately decompose the emission line profiles into multiple narrow components (FWHM ∼ 30-130 km s -1 ) superimposed on a broad (FWHM ∼ 150-350 km s -1 ) feature. This paper is the first of a series examining the optical structure of M82's disk and inner wind; here we focus on the ionized gaseous and stellar dynamics and present maps of the relevant emission line properties. Our observations show that ionized gas in the starburst core of M82 is dynamically complex with many overlapping expanding structures located at different radii. Localised line splitting of up to 100 km s -1 in the narrow component is associated with expanding shells of compressed, cool, photoionized gas at the roots of the superwind outflow. We have been able to associate some of this inner-wind gas with a distinct outflow channel characterised by its dynamics and gas density patterns, and we discuss the consequences of this discovery in terms of the developing wind outflow. The broad optical emission line component is observed to become increasingly important moving outward along the outflow channel, and in general with increasing height above/below the plane. Following our recent work on the origins of this component, we associate it with turbulent gas in wind-clump interface layers and hence sites of mass loading, meaning that the turbulent mixing of cooler gas into the outflowing hot gas must become increasingly important with height, and provides powerful direct evidence for the existence of mass-loading over a large, spatially extended area reaching far into the inner wind. We discuss the consequences and implications of this. We confirm
Radio emission from symbiotic stars: a binary model
International Nuclear Information System (INIS)
Taylor, A.R.; Seaquist, E.R.
1985-01-01
The authors examine a binary model for symbiotic stars to account for their radio properties. The system is comprised of a cool, mass-losing star and a hot companion. Radio emission arises in the portion of the stellar wind photo-ionized by the hot star. Computer simulations for the case of uniform mass loss at constant velocity show that when less than half the wind is ionized, optically thick spectral indices greater than +0.6 are produced. Model fits to radio spectra allow the binary separation, wind density and ionizing photon luminosity to be calculated. They apply the model to the symbiotic star H1-36. (orig.)
Inner-shell near-threshold photoionization of A-C60 endohedral atoms
International Nuclear Information System (INIS)
Baltenkov, Arkadiy S.; Dolmatov, Valery K.; Manson, Steven T.
2002-01-01
Photoelectron angular distributions and total photoionization cross sections of near-threshold 1s photoionization of Li from the oriented-in-space endohedral Li-C 60 fullerene are investigated within the framework of our recently developed photoionization theory of multicenter formations. Both at-the-center and off-the-center endohedral Li are considered, and off-the-center effects are shown to be of extreme importance, in contrast to the conventional wisdom. Multiple-scattering effects on the outgoing photoelectron are included and found to influence the photoionization spectra strongly, e.g., decreasing the cross section by more than an order of magnitude in certain cases, as compared to the situation when such effects are neglected. Diffraction resonances in the photoionization cross section of the endohedral Li atom are found as a result of the multicenter nature of the C 60 surrounding cage, and these are compared with the results of other empirical and ab initio theories. Since there is nothing particularly special about Li 1s with respect to photoionization, the trends uncovered in this paper should qualitatively apply to near-threshold inner-shell ns photoionization spectra of virtually any endohedral atom A from any A-C 60 endohedral fullerene formation
The effect of photoionizing feedback on star formation in isolated and colliding clouds
Shima, Kazuhiro; Tasker, Elizabeth J.; Federrath, Christoph; Habe, Asao
2018-05-01
We investigate star formation occurring in idealized giant molecular clouds, comparing structures that evolve in isolation versus those undergoing a collision. Two different collision speeds are investigated and the impact of photoionizing radiation from the stars is determined. We find that a colliding system leads to more massive star formation both with and without the addition of feedback, raising overall star formation efficiencies (SFE) by a factor of 10 and steepening the high-mass end of the stellar mass function. This rise in SFE is due to increased turbulent compression during the cloud collision. While feedback can both promote and hinder star formation in an isolated system, it increases the SFE by approximately 1.5 times in the colliding case when the thermal speed of the resulting H II regions matches the shock propagation speed in the collision.
Photoionization and vacancy decay of endohedral atoms
International Nuclear Information System (INIS)
Amusia, M. Ya.
2007-01-01
We demonstrate the role played by the fullerenes shell in the photoionization and vacancy decay of endohedral atoms A-C 60 . It is shown, partly in the frame of a rather simple model that describes the fullerene shell, partly using only the assumption on the smallness of the atom A in comparison to the size of C 60 that it affects photoionization and the vacancy decay of A-C 60 profoundly. Namely, it leads to a number of new resonances in photoionization cross-section and other photoionization characteristics as well as strong modifications of the vacancy decay probabilities and to opening of new decay channels. We will discuss the problem of photon propagation through the C 60 shell and conclude that at any considered frequency ω, 0 ≤ ω ≤ 60 eV the C 60 enhances the incoming radiation. This shows non-metallic dielectric behavior of the 240 collectivized electrons in C 60 . We also discuss the effects of C 60 upon the fast electron inelastic scattering. The results obtained are valid qualitatively also for other than C 60 molecules, e.g. for C 70 or C 76
Photoionization and vacancy decay of endohedral atoms
Energy Technology Data Exchange (ETDEWEB)
Amusia, M. Ya. [Racah Institute of Physics, Hebrew University, Jerusalem 91904 (Israel); A.F. Ioffe Physical-Technical Institute, St. Petersburg 194021 (Russian Federation)], E-mail: amusia@vms.huji.ac.il
2007-10-15
We demonstrate the role played by the fullerenes shell in the photoionization and vacancy decay of endohedral atoms A-C{sub 60}. It is shown, partly in the frame of a rather simple model that describes the fullerene shell, partly using only the assumption on the smallness of the atom A in comparison to the size of C{sub 60} that it affects photoionization and the vacancy decay of A-C{sub 60} profoundly. Namely, it leads to a number of new resonances in photoionization cross-section and other photoionization characteristics as well as strong modifications of the vacancy decay probabilities and to opening of new decay channels. We will discuss the problem of photon propagation through the C{sub 60} shell and conclude that at any considered frequency {omega}, 0 {<=} {omega} {<=} 60 eV the C{sub 60} enhances the incoming radiation. This shows non-metallic dielectric behavior of the 240 collectivized electrons in C{sub 60}. We also discuss the effects of C{sub 60} upon the fast electron inelastic scattering. The results obtained are valid qualitatively also for other than C{sub 60} molecules, e.g. for C{sub 70} or C{sub 76}.
International Nuclear Information System (INIS)
Breus, T.K.; Krymskij, A.M.; Mitnitskij, V.Ya.
1987-01-01
Numeric modelling of the Venus flow-around by the solar wind with regard to stream loading by heavy ions, produced under photoionization of the Venus neutral oxygen corona, is conducted. It is shown, that this effect can account for a whole number of peculiarities related to the solar wind interaction with the planet which have not been clearly explained yet, namely, shock wave position, solar wind stream and magnetic field characteristics behind the front
The Local ISM and its Interaction with the Winds of Nearby Late-type Stars
Wood, Brian E.; Linsky, Jeffrey L.
1998-01-01
We present new Goddard High-Resolution Spectrograph (GHRS) observations of the Ly-alpha and Mg II absorption lines seen toward the nearby stars 61 Cyg A and 40 Eri A. We use these data to measure interstellar properties along these lines of sight and to search for evidence of circumstellar hydrogen walls, which are produced by collisions between the stellar winds and the Local InterStellar Medium (LISM). We were able to model the Ly-alpha lines of both stars without hydrogen-wall absorption components, but for 61 Cyg A the fit required a stellar Ly-alpha, line profile with an improbably deep self-reversal, and for 40 Eri A the fit required a very low deuterium-to-hydrogen ratio that is inconsistent with previous GHRS measurements. Since these problems could be rectified simply by including stellar hydrogen-wall components with reasonable attributes, our preferred fits to the data include these components. We have explored several ways in which the hydrogen-wall properties measured here and in previous work can be used to study stellar winds and the LISM. We argue that the existence of a hydrogen wall around 40 Eri A and a low H I column density along that line of sight imply that either the interstellar density must decrease toward 40 Eri A or the hydrogen ionization fraction (chi) must increase. We find that hydrogen-wall temperatures are larger for stars with faster velocities through the LISM. The observed temperature-velocity relation is consistent with the predictions of hydromagnetic shock jump conditions. More precise comparison of the data and the jump conditions suggests crude upper limits for both chi and the ratio of magnetic to thermal pressure in the LISM (alpha): chi less than 0.6 and alpha less than 2. The latter upper limit corresponds to a limit on the LISM magnetic field of B less than 5 micro G. These results imply that the plasma Mach number of the interstellar wind flowing into the heliosphere is M(sub A) greater than 1.3, which indicates that
Effects of relativistic small radial component on atomic photoionization cross sections
International Nuclear Information System (INIS)
Liu Xiaobin; Xing Yongzhong; Sun Xiaowei
2008-01-01
The effects of relativistic small radial component on atomic photoionization cross sections have been studied within relativistic average self-consistent field theory. Relativistic effects are relatively unimportant for low photon energy, along with a review of high-energy photoionization the relativistic effects are quite important. The effects of relativistic small radial component on photoionization process should show breakdown when the nuclear finite-size effects is taken into account. The compression of wavefunction into the space near nucleus is so strong in highly charged ions that the electronic radius greatly decreases, and the effects of relativistic small radial component on photoionization cross sections turn to stronger than ordinary atoms. Since relativistic effects are extremely sensitive to the behavior of small radial component, the results are in good agreement with relativistic effects on photoionization cross section. (authors)
Study of Photoionization and Fragmentation on CHClF2 : Experiments and Calculations
International Nuclear Information System (INIS)
Sheng, L.; Yang, B.; Huang, C.; Qi, F.; Zhang, Y.; Wang, Z.; Zhou, S.
2004-01-01
Full text: The photoionization and fragmentation of CHClF 2 are studied with VUV radiation and photoionization mass spectroscopy at NSRL. Ionization potential of Parent molecule CHClF 2 , appearance energies of some fragment ions, and dissociative energy of some fragmentation process are obtained from photoionization efficiency spectroscopy. Dissociative photoionization channels for formation of some fragment ions are proposed on comparison of determined appearance energies and energies predicted with Gaussian-98 calculation
Absolute photoionization cross-section measurements of the Kr I isoelectronic sequence
International Nuclear Information System (INIS)
Kilbane, D.; Banahan, C.; Kampen, P. van; Costello, J. T.; Folkmann, F.; Kjeldsen, H.; Bizau, J.-M.; Scully, S.; Mansfield, M. W. D.; West, J. B.
2007-01-01
Photoionization spectra have been recorded in the 4s, 4p, and 3d resonance regions for the Kr I isoelectronic sequence using both the dual laser produced plasma (DLP) technique (at DCU) to produce photoabsorption spectra, and the merged ion beam and synchrotron radiation technique (at ASTRID) to measure absolute photoionization cross sections. Profile parameters are compared for the 4s-np resonances of Rb + and Sr 2+ . Many 4p→ns, md transitions are identified with the aid of Hartree-Fock calculations, and consistent quantum defects are observed for the various ns and md Rydberg series. Absolute single and double photoionization cross sections recorded in the 3d region for Rb + and Sr 2+ ions show preferential decay via double photoionization. This is only the second report to our knowledge where both the DLP technique and the merged-beam technique have been used simultaneously to record photoionization spectra, and the advantages of both techniques (i.e., better resolution in the case of DLP and values for absolute photoionization cross sections in the case of the merged-beam technique) are highlighted
Photoionization and electron-ion recombination of Cr I
International Nuclear Information System (INIS)
Nahar, Sultana N.
2009-01-01
Using the unified method, the inverse processes of photoionization and electron-ion recombination are studied in detail for neutral chromium, (CrI+hν↔CrII+e), for the ground and excited states. The unified method based on close-coupling approximation and R-matrix method (i) subsumes both the radiative recombination (RR) and dielectronic recombination (DR) for the total rate and (ii) provides self-consistent sets of photoionization cross sections σ PI and recombination rates α RC . The present results show in total photoionization of the ground and excited states an enhancement in the background at the first excited threshold, 3d 4 4s 5 D state of the core. One prominent phot-excitation-of-core (PEC) resonance due to one dipole allowed transition ( 6 S- 6 P o ) in the core is found in the photoionization cross sections of most of the valence electron excited states. Structures in the total and partial photoionization, for ionization into various excited core states and ground state only, respectively, are demonstrated. Results are presented for the septet and quintet states with n≤10 and l≤9 of Cr I. These states couple to the core ground state 6 S and contribute to the recombination rates. State-specific recombination rates are also presented for these states and their features are illustrated. The total recombination rate shows two DR peaks, one at a relatively low temperature, at 630 K, and the other around 40,000 K. This can explain existence of neutral Cr in interstellar medium. Calculations were carried out in LS coupling using a close-coupling wave function expansion of 40 core states. The results illustrate the features in the radiative processes of Cr I and provide photoionization cross sections and recombination rates with good approximation for this astrophysically important ion.
MAGNETIC NESTED-WIND SCENARIOS FOR BIPOLAR OUTFLOWS: PREPLANETARY AND YSO NEBULAR SHAPING
International Nuclear Information System (INIS)
Dennis, Timothy J.; Frank, Adam; Blackman, Eric G.; DeMarco, Orsola; Balick, Bruce; Mitran, Sorin
2009-01-01
We present results of a series of magnetohydrodynamic (MHD) and hydrodynamic (HD) 2.5 dimensional simulations of the morphology of outflows driven by nested wide-angle winds, i.e., winds that emanate from a central star as well as from an orbiting accretion disk. While our results are broadly relevant to nested-wind systems, we have tuned the parameters of the simulations to touch on issues in both young stellar objects and planetary nebula (PN) studies. In particular, our studies connect to open issues in the early evolution of PNs. We find that nested MHD winds exhibit marked morphological differences from the single MHD wind case along both dimensions of the flow. Nested HD winds, on the other hand, give rise mainly to geometric distortions of an outflow that is topologically similar to the flow arising from a single stellar HD wind. Our MHD results are insensitive to changes in ambient temperature between ionized and un-ionized circumstellar environments. The results are sensitive to the relative mass-loss rates and the relative speeds of the stellar and disk winds. We also present synthetic emission maps of both nested MHD and HD simulations. We find that nested MHD winds show knots of emission appearing on-axis that do not appear in the HD case.
A vacuum ultraviolet photoionization mass spectrometric study of acetone.
Wei, Lixia; Yang, Bin; Yang, Rui; Huang, Chaoqun; Wang, Jing; Shan, Xiaobin; Sheng, Liusi; Zhang, Yunwu; Qi, Fei; Lam, Chow-Shing; Li, Wai-Kee
2005-05-19
The photoionization and dissociative photoionization of acetone have been studied at the photon energy range of 8-20 eV. Photoionization efficiency spectra for ions CH3COCH3+, CH3+, C2H3+, C3H3+, C3H5+, CH(2-)CO+, CH3CO+, C3H4O+, and CH3COCH2+ have been measured. In addition, the energetics of the dissociative photoionization has been examined by ab initio Gaussian-3 (G3) calculations. The computational results are useful in establishing the dissociation channels near the ionization thresholds. With the help of G3 results, the dissociation channels for the formation of the fragment ions CH3CO+, CH2CO+, CH3+, C3H3+, and CH3COCH2+ have been established. The G3 results are in fair to excellent agreement with the experimental data.
Pindzola, M. S.; Abdel-Naby, Sh. A.; Robicheaux, F.; Colgan, J.
2014-05-01
Single and double photoionization cross sections for Ne8+ are calculated using a non-perturbative fully relativistic time-dependent close-coupling method. A Bessel function expansion is used to include both dipole and quadrupole effects in the radiation field interaction and the repulsive interaction between electrons includes both the Coulomb and Gaunt interactions. The fully correlated ground state of Ne8+ is obtained by solving a time-independent inhomogeneous set of close-coupled equations. Propagation of the time-dependent close-coupled equations yields single and double photoionization cross sections for Ne8+ at energies easily accessible at advanced free electron laser facilities. This work was supported in part by grants from NSF and US DoE. Computational work was carried out at NERSC in Oakland, California, NICS in Knoxville, Tennessee, and OLCF in Oak Ridge, Tennessee.
Dynamics of photoionization of hydrogenlike ions in Debye plasmas
International Nuclear Information System (INIS)
Qi, Y. Y.; Wang, J. G.; Janev, R. K.
2009-01-01
Photoionization processes for the ground state and n≤3 excited states of hydrogenlike ions embedded in a weakly coupled plasma are investigated in the entire energy range of a nonrelativistic regime. The plasma screening of the Coulomb interaction between charged particles is described by the Debye-Hueckel model. The energy levels and wave functions for both the bound and continuum states are calculated by solving the Schroedinger equation numerically by the symplectic integrator. The screening of Coulomb interactions reduces the number of bound electron states, decreases their binding energies, broadens the radial distribution of electron wave functions of these states, and changes significantly the phases and the amplitudes of continuum wave functions. These changes strongly affect the dipole matrix elements between the bound and continuum states and, hence, the photoionization cross sections. The most significant effects of the screened Coulomb interactions on the energy behavior of photoionization cross sections are manifested in its low-energy behavior (Wigner threshold law), the appearance of multiple shape and virtual-state resonances when the energy levels of upper bound states enter the continuum after certain critical strength of the screening, and in the (slight) reduction of the cross section at high photon energies. All these features of the photoionization cross section are related to the short-range character of the Debye-Hueckel potential. The effects of the potential screening on the Combet-Farnoux and Cooper minima in the photoionization cross section are also investigated. Comparison of calculated photoionization cross sections with the results of other authors, when available, is made.
Surface states in the photoionization of high-quality CdSe core/shell nanocrystals.
Li, Shu; Steigerwald, Michael L; Brus, Louis E
2009-05-26
We use electric force microscopy (EFM) to study single nanocrystal photoionization in two classes of high-quality nanocrystals whose exciton luminescence quantum yields approach unity in solution. The CdSe/CdS/ZnS core/shell nanocrystals do not photoionize, while the CdSe/CdS nanocrystals do show substantial photoionization. This verifies the theoretical prediction that the ZnS shell confines the excited electron within the nanocrystal. Despite the high luminescence quantum yield, photoionization varies substantially among the CdSe/CdS nanocrystals. We have studied the nanocrystal photoionization with both UV (396 nm) and green (532 nm) light, and we have found that the magnitude of the charge due to photoionization per absorbed photon is greater for UV excitation than for green excitation. A fraction of the photoionization occurs directly via a "hot electron" process, using trap states that are either on the particle surface, within the ligand sphere, or within the silicon oxide layer. This must occur without relaxation to the thermalized, lowest-energy, emitting exciton. We discuss the occurrence of hot carrier processes that are common to photoionization, luminescence blinking, and the fast transient optical absorption that is associated with multiple exciton generation MEG studies.
Radio continuum emission from young stellar objects in L1641
International Nuclear Information System (INIS)
Morgan, J.A.; Snell, R.L.; Strom, K.M.
1990-01-01
The results of a 6 and 20 cm radio continuum survey of young stellar objects in the L1641 region located south of the Orion Nebula are presented. Four are identified as low-luminosity young stellar objects in L1641 and three more as Herbig-Haro or Herbig-Haro-like objects. These objects have bolometric luminosities between 80 and 300 solar, and their 6-20 cm spectral index suggests optically thick, free-free emission. They are characterized by a rising spectrum between 2.2 and 25 microns, have no optical counterparts, and are associated with stellar wind activity. Thus, detectable radio continuum emission may be produced only by the youngest and most luminous objects in L1641. 34 refs
Component manufacturing development for the National Compact Stellarator Experiment (NCSX)
International Nuclear Information System (INIS)
Heitzenroeder, P.J.; Brown, T.G.; Chrzanowski, J.H.; Neilson, G.H.; Reiersen, W.T.; Sutton, L.L.; Viola, M.E.; Cole, M.J.; Goranson, P.L.; Nelson, B.E.; Williamson, D.E.
2005-01-01
NCSX is the first of a new class of stellarators called compact stellarators which hold the promise of retaining the steady state feature of the stellarator but at a much lower aspect ratio and using a quasi-axisymmetric magnetic field to obtain tokamak-like performance. Although much of NCSX is conventional in design and construction, the vacuum vessel and modular coils provide significant engineering challenges due to their complex shapes, need for high dimensional accuracy, and the need for high current density in the modular coils due space constraints. Consequently, a three-phase development program has been undertaken. In the first phase, laboratory / industrial studies were performed during the development of the conceptual design to permit advances in manufacturing technology to be incorporated into NCSX's plans. In the second phase, full-scale prototype modular coil winding forms, compacted cable conductors, and 20-degree sectors of the vacuum vessel were fabricated in industry. In parallel, the NCSX project team undertook R and D studies that focused on the windings. The third (production) phase began in September 2004. First plasma is scheduled for January 2008. (author)
Photoionization of excited molecular states using multiphoton excitation techniques
International Nuclear Information System (INIS)
Dehmer, P.M.; Pratt, S.T.; Dehmer, J.L.
1984-01-01
Photoelectron spectra are reported for three photon resonant, four photon ionization of H 2 via the B 1 Σ + /sub u/, v = 7 (J = 2,4) and C 1 Pi/sub u/, v = 0-4 (J = 1) levels and of N 2 via the o 3 1 Pi/sub u/, v = 1,2, b 1 Pi/sub u/, v = 3-5, and c 1 Pi/sub u/, v = 0 levels. The results reflect both the spectroscopy and the dynamics of photoionization of excited molecular states and are discussed in terms of the selection rules for photoionization and the relative probabilities of photoionization from Rydberg and valence states. In some cases, in accordance with the Franck-Condon principle, the results demonstrate that resonant multiphoton ionization through Rydberg states may be a powerful technique for the production of electronic, vibrational, and rotational state selected ions. However, in other cases, systematic departures from Franck-Condon factors are observed, which reflect the more subtle dynamics of excited state photoionization
Molecular beam photoionization and gas-surface scattering
International Nuclear Information System (INIS)
Ceyer, S.T.
1979-09-01
The energetics of the ethylene ion-molecule reactions was investigated in more detail than previously possible in two body collision experiments by photoionization of the neutral van der Waals ethylene dimer. The stability of the (C 2 H 4 ) + C 2 H 4 ion-molecule collision complex has been determined to be 18.2 +- 0.5 kcal. The highest potential barriers along the reaction coordinate for decomposition of this collision complex into C 4 H 7 + + H and C 3 H 5 + + CH 3 have been determined to be 0 +- 1.5 and 8.7 +- 1.5 kcal. In a similar manner, the energetics of the solvated ethylene dimer ion was investigated by the photoionization of the ethylene trimer. The absolute proton affinity of NH 3 (203.6 +- 1.3 kcal/mole) and the proton solvation energies by more than one NH 3 have been determined by molecular beam photoionization. In addition, the NH 3 + -NH 3 interaction energy (0.79 +- 0.05 eV) was measured by photoionization of the neutral van der Waals dimer. These experiments have shown that photoionization of van der Waals clusters is a very powerful method of determining the energetics of gas phase proton solvation. The scattering of helium atomic beams from a high Miller index platinum surface that exhibits ordered, periodic steps on the atomic scale to probe the effect of atomic steps on the scattering distribution is explored. Rainbow scattering is observed when the step edges are perpendicular to the incident helium atoms. The design, construction and operation of a beam-surface scattering apparatus are described. The first data obtained in this apparatus are presented and the interesting dynamical aspects of the oxidation of D, D 2 and CO are discussed. 75 references
International Nuclear Information System (INIS)
Liu Mengmeng; Ma Xiaoguang
2011-01-01
The conversion rules under which an algebraic expression can be obtained from a corresponding photoionization Goldstone diagram have been given systematically in the present work. The electronic correlations in the photoionization processes then could be studied diagrammatically. The application to atomic scandium shows that the present theoretical scheme can give reasonable photoionization cross sections, which agree well with the experimental results. (atomic and molecular physics)
Photoionization of multiply charged ions at the advanced light source
International Nuclear Information System (INIS)
Schlachter, A.S.; Kilcoyne, A.L.D.; Aguilar, A.; Gharaibeh, M.F.; Emmons, E.D.; Scully, S.W.J.; Phaneuf, R.A.; Muller, A.; Schippers, S.; Alvarez, I.; Cisneros, C.; Hinojosa, G.; McLaughlin, B.M.
2004-01-01
Photoionization of multiply charged ions is studied using the merged-beams technique at the Advanced Light Source. Absolute photoionization cross sections have been measured for a variety of ions along both isoelectronic and isonuclear sequences
Combination of lasers and synchrotron radiation in studies of atomic photoionization
International Nuclear Information System (INIS)
Meyer, M.
2009-01-01
Recent experiments using the combination of conventional lasers and synchrotron radiation are presented and discussed. The controlled laser-manipulation of atoms prior to ionization by the synchrotron radiation provides an ideal experimental basis for detailed investigations of atomic photoionization. Due to the recent advances in high-resolution electron spectroscopy, it has become possible to analyze the J-resolved fine structure of the final ionic states in the photoionization of laser-excited atoms enabling thereby the determination of the specific influence of the outer electron to the ionization from inner subshells. Especially, the analysis of photoemission satellites and their relative intensities bring out directly the importance of electron correlations. Furthermore, it is shown through some examples of experiments using linearly and circularly polarized radiations, how the study of magnetic dichroisms in the photoionization opens the access to a complete description of the photoionization process, in particular to the determination of partial photoionization cross-sections.
Dissociative photoionization of 1,3-butadiene: experimental and theoretical insights.
Fang, Wenzheng; Gong, Lei; Zhang, Qiang; Shan, Xiaobin; Liu, Fuyi; Wang, Zhenya; Sheng, Liusi
2011-05-07
The vacuum-ultraviolet photoionization and dissociative photoionization of 1,3-butadiene in a region ∼8.5-17 eV have been investigated with time-of-flight photoionization mass spectrometry using tunable synchrotron radiation. The adiabatic ionization energy of 1,3-butadiene and appearance energies for its fragment ions, C(4)H(5)(+), C(4)H(4)(+), C(4)H(3)(+), C(3)H(3)(+), C(2)H(4)(+), C(2)H(3)(+), and C(2)H(2)(+), are determined to be 9.09, 11.72, 13.11, 15.20, 11.50, 12.44, 15.15, and 15.14 eV, respectively, by measurements of photoionization efficiency spectra. Ab initio molecular orbital calculations have been performed to investigate the reaction mechanism of dissociative photoionization of 1,3-butadiene. On the basis of experimental and theoretical results, seven dissociative photoionization channels are proposed: C(4)H(5)(+) + H, C(4)H(4)(+) + H(2), C(4)H(3)(+) + H(2) + H, C(3)H(3)(+) + CH(3), C(2)H(4)(+) + C(2)H(2), C(2)H(3)(+) + C(2)H(2) + H, and C(2)H(2)(+) + C(2)H(2) + H(2). Channel C(3)H(3)(+) + CH(3) is found to be the dominant one, followed by C(4)H(5)(+) + H and C(2)H(4)(+) + C(2)H(2). The majority of these channels occur via isomerization prior to dissociation. Transition structures and intermediates for those isomerization processes were also determined.
Selectivity, specificity, and sensitivity in the photoionization of sputtered species
International Nuclear Information System (INIS)
Gruen, D.M.; Calaway, W.F.; Pellin, M.J.; Young, C.E.; Spiegel, D.R.; Clayton, R.N.; Davis, A.M.; Blum, J.D.
1990-01-01
To deal with the problem of non- or near-resonant ionization, one needs to achieve the highest selectively for photoionization of the species of interest relative to isobarically overlapping species by choosing a specific photoionization scheme tailoring are that is could not have near-overlap with known atomic or molecular energy levels of isobaric species, and that it should lead to saturation of the resonance transitions at the lowest possible laser power levels so as to minimize two- and three-photon nonresonant photoionization processes. Experience has shown that, even when these two conditions are met as closely as possible, non- or near-resonant ionization can still occur, perhaps because of the existence of hitherto unobserved energy levels, photodissociation of sputtered molecules, or other effects. It is becoming clear that maximizing detection sensitivity for a particular species requires one to pay careful attention to the selection of an optimal photoionization scheme. It is the purpose of the present paper to illustrate this point with several examples and to help point the way to still further improvements in detection sensitivity by non- or near-resonant. ionization through detailed exploration of alternative photoionization schemes
TIDALLY ENHANCED STELLAR WIND: A WAY TO MAKE THE SYMBIOTIC CHANNEL TO TYPE Ia SUPERNOVA VIABLE
International Nuclear Information System (INIS)
Chen, X.; Han, Z.; Tout, C. A.
2011-01-01
In the symbiotic (or WD+RG) channel of the single-degenerate scenario for type Ia supernovae (SNe Ia), the explosions occur a relatively long time after star formation. The birthrate from this channel would be too low to account for all observed SNe Ia were it not for some mechanism to enhance the rate of accretion on to the white dwarf. A tidally enhanced stellar wind, of the type which has been postulated to explain many phenomena related to giant star evolution in binary systems, can do this. Compared to mass stripping, this model extends the space of SNe Ia progenitors to longer orbital periods and hence increases the birthrate to about 0.0069 yr -1 for the symbiotic channel. Two symbiotic stars, T CrB and RS Oph, considered to be the most likely progenitors of SNe Ia through the symbiotic channel, are well inside the period-companion mass space predicted by our models.
Vacuum ultraviolet photoionization cross section of the hydroxyl radical.
Dodson, Leah G; Savee, John D; Gozem, Samer; Shen, Linhan; Krylov, Anna I; Taatjes, Craig A; Osborn, David L; Okumura, Mitchio
2018-05-14
The absolute photoionization spectrum of the hydroxyl (OH) radical from 12.513 to 14.213 eV was measured by multiplexed photoionization mass spectrometry with time-resolved radical kinetics. Tunable vacuum ultraviolet (VUV) synchrotron radiation was generated at the Advanced Light Source. OH radicals were generated from the reaction of O( 1 D) + H 2 O in a flow reactor in He at 8 Torr. The initial O( 1 D) concentration, where the atom was formed by pulsed laser photolysis of ozone, was determined from the measured depletion of a known concentration of ozone. Concentrations of OH and O( 3 P) were obtained by fitting observed time traces with a kinetics model constructed with literature rate coefficients. The absolute cross section of OH was determined to be σ(13.436 eV) = 3.2 ± 1.0 Mb and σ(14.193 eV) = 4.7 ± 1.6 Mb relative to the known cross section for O( 3 P) at 14.193 eV. The absolute photoionization spectrum was obtained by recording a spectrum at a resolution of 8 meV (50 meV steps) and scaling to the single-energy cross sections. We computed the absolute VUV photoionization spectrum of OH and O( 3 P) using equation-of-motion coupled-cluster Dyson orbitals and a Coulomb photoelectron wave function and found good agreement with the observed absolute photoionization spectra.
Vacuum ultraviolet photoionization cross section of the hydroxyl radical
Dodson, Leah G.; Savee, John D.; Gozem, Samer; Shen, Linhan; Krylov, Anna I.; Taatjes, Craig A.; Osborn, David L.; Okumura, Mitchio
2018-05-01
The absolute photoionization spectrum of the hydroxyl (OH) radical from 12.513 to 14.213 eV was measured by multiplexed photoionization mass spectrometry with time-resolved radical kinetics. Tunable vacuum ultraviolet (VUV) synchrotron radiation was generated at the Advanced Light Source. OH radicals were generated from the reaction of O(1D) + H2O in a flow reactor in He at 8 Torr. The initial O(1D) concentration, where the atom was formed by pulsed laser photolysis of ozone, was determined from the measured depletion of a known concentration of ozone. Concentrations of OH and O(3P) were obtained by fitting observed time traces with a kinetics model constructed with literature rate coefficients. The absolute cross section of OH was determined to be σ(13.436 eV) = 3.2 ± 1.0 Mb and σ(14.193 eV) = 4.7 ± 1.6 Mb relative to the known cross section for O(3P) at 14.193 eV. The absolute photoionization spectrum was obtained by recording a spectrum at a resolution of 8 meV (50 meV steps) and scaling to the single-energy cross sections. We computed the absolute VUV photoionization spectrum of OH and O(3P) using equation-of-motion coupled-cluster Dyson orbitals and a Coulomb photoelectron wave function and found good agreement with the observed absolute photoionization spectra.
Energy Technology Data Exchange (ETDEWEB)
Khodachenko, M. L.; Lammer, H.; Kislyakova, K. G.; Fossati, L.; Arkhypov, O. V. [Space Research Institute, Austrian Academy of Sciences, Graz (Austria); Shaikhislamov, I. F.; Berezutsky, A. G.; Miroshnichenko, I. B.; Posukh, V. G. [Institute of Laser Physics SB RAS, Novosibirsk (Russian Federation); Johnstone, C. P., E-mail: maxim.khodachenko@oeaw.ac.at [Department of Astrophysics, University of Vienna (Austria)
2017-10-01
To shed more light on the nature of the observed Ly α absorption during transits of HD 209458b and to quantify the major mechanisms responsible for the production of fast hydrogen atoms (the so-called energetic neutral atoms, ENAs) around the planet, 2D hydrodynamic multifluid modeling of the expanding planetary upper atmosphere, which is driven by stellar XUV, and its interaction with the stellar wind has been performed. The model self-consistently describes the escaping planetary wind, taking into account the generation of ENAs due to particle acceleration by the radiation pressure and by the charge exchange between the stellar wind protons and planetary atoms. The calculations in a wide range of stellar wind parameters and XUV flux values showed that under typical Sun-like star conditions, the amount of generated ENAs is too small, and the observed absorption at the level of 6%–8% can be attributed only to the non-resonant natural line broadening. For lower XUV fluxes, e.g., during the activity minima, the number of planetary atoms that survive photoionization and give rise to ENAs increases, resulting in up to 10%–15% absorption at the blue wing of the Ly α line, caused by resonant thermal line broadening. A similar asymmetric absorption can be seen under the conditions realized during coronal mass ejections, when sufficiently high stellar wind pressure confines the escaping planetary material within a kind of bowshock around the planet. It was found that the radiation pressure in all considered cases has a negligible contribution to the production of ENAs and the corresponding absorption.
Two-color photoionization and photoelectron studies by combining infrared and vacuum ultraviolet
International Nuclear Information System (INIS)
Ng, C.Y.
2005-01-01
Recent developments of two-color infrared (IR)-vacuum ultraviolet (VUV) and VUV-IR photoionization and photoelectron detection schemes for spectroscopic studies are described. By preparing molecules in selected rovibrational states by IR excitation prior to VUV-photoionization, state-selected and state-to-state photoionization cross sections can be obtained by IR-VUV-photoionization efficiency (IR-VUV-PIE) and IR-VUV-pulsed field ionization-photoelectron (IR-VUV-PFI-PE) measurements, respectively. Rotationally resolved autoionizing Rydberg states converging to excited ionic states, which cannot be observed by single-photon VUV-PIE measurements, can be examined by the IR-VUV-PIE scheme. By monitoring the photoion and the PFI-PE intensities at a fixed VUV energy as a function of IR frequency, the respective IR photoion and IR absorption spectra of the corresponding neutral molecule can be measured. Two-color VUV-IR photo-induced Rydberg ionization (PIRI) experiment, in which high-n Rydberg states are prepared by VUV-photoexcitation followed by IR-induced autoionization, has also been demonstrated. Since the IR-VUV-PIE, IR-VUV-PFI-PE, and VUV-IR-PIRI methods do not require the existence of a bound intermediate electronic state in the UV and are generally applicable to all molecules, the development of these two-color photoionization and photoelectron schemes is expected to significantly enhance the scope of VUV spectroscopy and chemistry
Kislyakova, Kristina G; Lammer, Helmut; Holmström, Mats; Panchenko, Mykhaylo; Odert, Petra; Erkaev, Nikolai V; Leitzinger, Martin; Khodachenko, Maxim L; Kulikov, Yuri N; Güdel, Manuel; Hanslmeier, Arnold
2013-11-01
We studied the interactions between the stellar wind plasma flow of a typical M star, such as GJ 436, and the hydrogen-rich upper atmosphere of an Earth-like planet and a "super-Earth" with a radius of 2 R(Earth) and a mass of 10 M(Earth), located within the habitable zone at ∼0.24 AU. We investigated the formation of extended atomic hydrogen coronae under the influences of the stellar XUV flux (soft X-rays and EUV), stellar wind density and velocity, shape of a planetary obstacle (e.g., magnetosphere, ionopause), and the loss of planetary pickup ions on the evolution of hydrogen-dominated upper atmospheres. Stellar XUV fluxes that are 1, 10, 50, and 100 times higher compared to that of the present-day Sun were considered, and the formation of high-energy neutral hydrogen clouds around the planets due to the charge-exchange reaction under various stellar conditions was modeled. Charge-exchange between stellar wind protons with planetary hydrogen atoms, and photoionization, lead to the production of initially cold ions of planetary origin. We found that the ion production rates for the studied planets can vary over a wide range, from ∼1.0×10²⁵ s⁻¹ to ∼5.3×10³⁰ s⁻¹, depending on the stellar wind conditions and the assumed XUV exposure of the upper atmosphere. Our findings indicate that most likely the majority of these planetary ions are picked up by the stellar wind and lost from the planet. Finally, we estimated the long-time nonthermal ion pickup escape for the studied planets and compared them with the thermal escape. According to our estimates, nonthermal escape of picked-up ionized hydrogen atoms over a planet's lifetime within the habitable zone of an M dwarf varies between ∼0.4 Earth ocean equivalent amounts of hydrogen (EO(H)) to <3 EO(H) and usually is several times smaller in comparison to the thermal atmospheric escape rates.
Lammer, Helmut; Holmström, Mats; Panchenko, Mykhaylo; Odert, Petra; Erkaev, Nikolai V.; Leitzinger, Martin; Khodachenko, Maxim L.; Kulikov, Yuri N.; Güdel, Manuel; Hanslmeier, Arnold
2013-01-01
Abstract We studied the interactions between the stellar wind plasma flow of a typical M star, such as GJ 436, and the hydrogen-rich upper atmosphere of an Earth-like planet and a “super-Earth” with a radius of 2 REarth and a mass of 10 MEarth, located within the habitable zone at ∼0.24 AU. We investigated the formation of extended atomic hydrogen coronae under the influences of the stellar XUV flux (soft X-rays and EUV), stellar wind density and velocity, shape of a planetary obstacle (e.g., magnetosphere, ionopause), and the loss of planetary pickup ions on the evolution of hydrogen-dominated upper atmospheres. Stellar XUV fluxes that are 1, 10, 50, and 100 times higher compared to that of the present-day Sun were considered, and the formation of high-energy neutral hydrogen clouds around the planets due to the charge-exchange reaction under various stellar conditions was modeled. Charge-exchange between stellar wind protons with planetary hydrogen atoms, and photoionization, lead to the production of initially cold ions of planetary origin. We found that the ion production rates for the studied planets can vary over a wide range, from ∼1.0×1025 s−1 to ∼5.3×1030 s−1, depending on the stellar wind conditions and the assumed XUV exposure of the upper atmosphere. Our findings indicate that most likely the majority of these planetary ions are picked up by the stellar wind and lost from the planet. Finally, we estimated the long-time nonthermal ion pickup escape for the studied planets and compared them with the thermal escape. According to our estimates, nonthermal escape of picked-up ionized hydrogen atoms over a planet's lifetime within the habitable zone of an M dwarf varies between ∼0.4 Earth ocean equivalent amounts of hydrogen (EOH) to stars—Early atmospheres—Earth-like exoplanets—Energetic neutral atoms—Ion escape—Habitability. Astrobiology 13, 1030–1048. PMID:24283926
The Disk Wind in the Rapidly Spinning Stellar-mass Black Hole 4U 1630-472 Observed with NuSTAR
King, Ashley L.; Walton, Dominic J.; Miller, Jon M.; Barret, Didier; Boggs, Steven E.; Christensen, Finn E.; Craig, William W.; Fabian, Andy C.; Furst, Felix; Hailey, Charles J.;
2014-01-01
We present an analysis of a short NuSTAR observation of the stellar-mass black hole and low-mass X-ray binary 4U 1630-472. Reflection from the inner accretion disk is clearly detected for the first time in this source, owing to the sensitivity of NuSTAR. With fits to the reflection spectrum, we find evidence for a rapidly spinning black hole, a* = 0.985(+0.005/-0.014) (1 sigma statistical errors). However, archival data show that the source has relatively low radio luminosity. Recently claimed relationships between jet power and black hole spin would predict either a lower spin or a higher peak radio luminosity. We also report the clear detection of an absorption feature at 7.03 +/- 0.03 keV, likely signaling a disk wind. If this line arises in dense, moderately ionized gas (log xi = 3.6(+0.2/-0.3) and is dominated by He-like Fe xxv, the wind has a velocity of v/c = 0.043(+0.002/-0.007) (12900(+600/-2100) km s(exp -1)). If the line is instead associated with a more highly ionized gas (log xi = 6.1(+0.7/-0.6)), and is dominated by Fe xxvi, evidence of a blueshift is only marginal, after taking systematic errors into account. Our analysis suggests the ionized wind may be launched within 200-1100 Rg, and may be magnetically driven.
Photoionization of Rydberg hydrogen atom in a magnetic field
International Nuclear Information System (INIS)
Wang, Dehua; Cheng, Shaohao; Chen, Zhaohang
2015-01-01
Highlights: • The ionization of Rydberg hydrogen atom in a magnetic field has been studied. • Oscillatory structures appear in the electron probability density distributions. • This study can guide the experimental research on the photoionization microscopy. - Abstract: The ionization of Rydberg hydrogen atom in a magnetic field has been studied on the basis of a semiclassical analysis of photoionization microscopy. The photoionization microscopy interference patterns of the photoelectron probability density distribution on a given detector plane are calculated at different scaled energies. We find that due to the interference effect of different types of electron trajectories arrived at a given point on the detector plane, oscillatory structures appear in the electron probability density distributions. The oscillatory structure of the interference pattern, which contains the spatial component of the electronic wave function, evolves sensitively on the scaled energy, through which we gain a deep understanding on the probability density distribution of the electron wave function. This study provides some reference values for the future experiment research on the photoionization microscopy of the Rydberg atom in the presence of magnetic field
Photoionization of excited molecular states using multiphoton excitation techniques
International Nuclear Information System (INIS)
Dehmer, P.M.; Pratt, S.T.; Dehmer, J.L.
1984-01-01
Photoelectron spectra are reported for three photon resonant, four photon ionization of H 2 via the B 1 Σ/sub u/ + , v = 7 (J = 2,4) and C 1 π/sub u'/, v = 0-4 (J = 1) levels and of N 2 via the o 3 1 π/sub u'/, v = 1,2, b 1 π/sub u'/, v = 3-5, and c 1 π/sub u'/, v = 0 levels. The results reflect both the spectroscopy and the dynamics of photoionization of excited molecular states and are discussed in terms of the selection rules for photoionization and the relative probabilities of photoionization from Rydberg and valence states. In some cases, in accordance with the Franck-Condon principle, the results demonstrate that resonant multiphoton ionization through Rydberg states may be a powerful technique for the production of electronic, vibrational, and rotational state selected ions. However, in other cases, systematic departures from Franck-Condon factors are observed, which reflect the more subtle dynamics of excited state photoionization. 23 references, 6 figures, 2 tables
The photoionization of the diffuse galactic gas
Mathis, J. S.
1986-01-01
In a study of the diffuse ionized gas (DIG) component of the interstellar medium, it is attempted to see if the general properties of dilute gas ionized by O stars are similar to observations and to what extent the observations of the DIG can be used to determine the nature of the ionizing radiation field at great distances above the plane of the Galaxy. It has been suggested by Reynolds (1985) that either shocks or photoionization might be responsible for the DIG. The photoionization model seems required by the observations.
Quadrupole photoionization of endohedral Xe-C60
International Nuclear Information System (INIS)
Govil, Karan; Deshmukh, P C
2009-01-01
The effect of an endohedral confinement on the quadrupole photoionization of atomic Xe is studied using the relativistic random phase approximation (RRPA). The atom's confinement is modelled by placing atomic Xe at the centre of a C 60 cage represented by an annular potential around it. A new confinement resonance is reported in the 4p quadrupole cross-section along with 'correlation confinement resonances' in 4d, 5s and 5p photoionizations at about 185 eV. The effect of the confinement on the non-dipole photoelectron angular distribution parameter γ is also reported.
Photoionization from the 6p 2P3/2 state of neutral cesium
International Nuclear Information System (INIS)
Haq, S. U.; Nadeem, Ali
2010-01-01
We report the photoionization studies of cesium from the 6p 2 P 3/2 excited state to measure the photoionization cross section at and above the first ionization threshold, oscillator strength of the highly excited transitions, and extension in the Rydberg series. The photoionization cross section at the first ionization threshold is measured as 25 (4) Mb and at excess energies 0.02, 0.04, 0.07, and 0.09 eV as 21, 19, 17, and 16 Mb, respectively. Oscillator strength of the 6p 2 P 3/2 → nd 2 D 5/2 (23 ≤ n ≤ 60) Rydberg transitions has been extracted utilizing the threshold value of photoionization cross section and the recorded nd 2 D 5/2 photoionization spectra.
Schultz, David
As recognized prominently by the APRA program, interpretation of NASA astrophysical mission observations requires significant products of laboratory astrophysics, for example, spectral lines and transition probabilities, electron-, proton-, or heavy-particle collision data. Availability of these data underpin robust and validated models of astrophysical emissions and absorptions, energy, momentum, and particle transport, dynamics, and reactions. Therefore, measured or computationally derived, analyzed, and readily available laboratory astrophysics data significantly enhances the scientific return on NASA missions such as HST, Spitzer, and JWST. In the present work a comprehensive set of data will be developed for the ubiquitous proton-hydrogen and hydrogen-hydrogen collisions in astrophysical environments including ISM shocks, supernova remnants and bubbles, HI clouds, young stellar objects, and winds within stellar spheres, covering the necessary wide range of energy- and charge-changing channels, collision energies, and most relevant scattering parameters. In addition, building on preliminary work, a transport and reaction simulation will be developed incorporating the elastic and inelastic collision data collected and produced. The work will build upon significant previous efforts of the principal investigators and collaborators, will result in a comprehensive data set required for modeling these environments and interpreting NASA astrophysical mission observations, and will benefit from feedback from collaborators who are active users of the work proposed.
Photoionization in the halo of the Galaxy
Bregman, Joel N.; Harrington, J. Patrick
1986-01-01
The ionizing radiation field in the halo is calculated and found to be dominated in the 13.6-45 eV range by light from O-B stars that escapes the disk, by planetary nebulae at 45-54 eV, by quasars and the Galactic soft X-ray background at 54-2000 eV, and by the extragalactic X-ray background at higher energies. Photoionization models are calculated with this radiation field incident on halo clouds of constant density for a variety of densities, for normal and depleted abundances, and with variations of the incident spectrum. For species at least triply ionized, such as Si IV, C IV, N V, and O VI, the line ratios are determined by intervening gas with the greatest volume, which is not necessarily the greatest mass component. Column densities from doubly ionized species like Si III should be greater than from triply ionized species. The role of photoionized gas in cosmic ray-supported halos and Galactic fountains is discussed. Observational tests of photoionization models are suggested.
Champeaux, J.-P.; Moretto-Capelle, P.; Cafarelli, P.; Deville, C.; Sence, M.; Casta, R.
2014-06-01
The physical interactions of polycyclic aromatic hydrocarbons (PAHs) with stellar particular radiation are key to understanding the life cycle of PAHs, their abundance and their role in the complex astrochemistry of the interstellar medium. In this context, we present experimental results on the ionization/fragmentation of isolated coronene by a 100-keV proton, reproducing interactions between stellar winds and PAH molecules in the star's environment. In particular, we show, without ambiguity, that such ionization/fragmentation induces intense dehydrogenation processes for which the loss of even numbers of hydrogen atoms and the detection of CH_2+ cations as a possible H2 precursor strongly suggest the formation of H2 neutral molecules along a scenario revealed by a quantum chemical calculation. We have evaluated the H2 emission cross-section from the coronene/proton interaction at 100 and 1.6 keV to be 2.97 × 10-16 and 3.3 × 10-16 cm2, respectively. A qualitative discussion on the formation rate of H2 in the HD 44179 Red Rectangle (RR) nebula leads to the conclusion that such processes could be very efficient, especially inside planetary nebulae rich in PAH molecules interacting with high proton mass-loss rate stars (such as post-asymptotic giant branch stars) or high velocity jets produced by an accretion disc.
Mass-Selective Laser Photoionization.
Smalley, R. E.
1982-01-01
Discusses the nature and applications of mass-selective laser photoionization. The ionization can be done with a single intense laser pulse lasting a few billionths of a second with no molecular fragmentation. Applications focus on: (1) benzene clusters, excimers, and exciplexes; (2) metal clusters; and (3) triplet formation and decay. (Author/JN)
Photoionization of three isomers of the C9H7 radical.
Hemberger, Patrick; Steinbauer, Michael; Schneider, Michael; Fischer, Ingo; Johnson, Melanie; Bodi, Andras; Gerber, Thomas
2010-04-15
Three resonance-stabilized radicals, 1-indenyl (Ind), 1-phenylpropargyl (1PPR), and 3-phenylpropargyl (3PPR), all isomers of the composition C(9)H(7), were generated by jet flash pyrolysis. Their photoionization was examined by VUV synchrotron radiation. The mass spectra show a clean and efficient radical generation when the pyrolysis is turned on. To study the photoionization, photoion yield measurements and threshold photoionization spectroscopy techniques were applied. We determined adiabatic ionization energies (IE(ad)) of 7.53 eV for Ind, 7.20 eV for 3PPR, and 7.4 eV for 1PPR. Ab initio calculations show no major change in geometry upon ionization, in agreement with ionization from a nonbonding molecular orbital. The IEs were also computed and are in agreement with the measured ones. The difference in the IE might allow a distinction of the three isomers in flames. In the indenyl spectrum, an excited a(+) (3)B(2) state of the cation was identified at 8.10 eV, which shows a low-energy vibrational progression of 61 meV. Furthermore, we have examined the dissociative photoionization of the precursors. The indenyl precursor, 1-indenyl bromide, undergoes dissociative photoionization to Ind(+). An appearance energy (AE(0K)) of 10.2 eV was obtained from fitting the experimental breakdown diagram. A binding energy of 1.8 eV can thus be determined for the C-Br bond in 1-indenyl bromide. The phenylpropargyl precursors 1PPBr (1-phenylpropargyl bromide/3-phenyl-3-bromopropyne) and 3PPBr (3-phenylpropargyl bromide/1-phenyl-3-bromopropyne) also lose a bromine atom upon dissociative photoionization. Approximate appearance energies of 9.8 eV for 3PPBr and 9.3 eV for 1PPBr have been determined.
High sensitivity detection of desorbed biomolecules by photoionization with tunable VUV
International Nuclear Information System (INIS)
Moore, J.F.; Calaway, W.F.; Veryovkin, I.V.; Pellin, M.J.; Lewellen, J.W.; Li, Y.; Milton, S.V.; King, B.V.
2004-01-01
Full text: The spectral region from 7 to 11eV has two attributes that make it attractive for biomolecule photoionization: 1. high photoionization cross sections, leading to high detection efficiency, and 2. overlap with nearly all first ionization energies of biomolecules, allowing possible control over fragmentation by accessing different final states via tuning. The lack of available tunable lasers in this energy range has generally hindered exploitation of these features thus far. A free-electron laser in operation at Argonne National Laboratory provides high pulse energy, widely tunable VUV pulses of 300 fs duration. Coupled with a novel time-of-flight mass spectrometer, this laser is able to photoionize and detect biomolecules, including peptides and nucleosides. Either laser desorption or primary ion beams are used to desorb sample material, followed by photoionization with a VUV laser. The instrument uses novel ion optics to extract photoions from a large volume while maintaining high mass resolution. This approach is capable of yielding dramatically improved detection limits over more conventional methods such as MALDI and SIMS. In the case of the common peptide substance P, for example, a substantial improvement over the MALDI signal was observed using VUV photoionization with very little observed fragmentation of the molecule. Nucleosides and cisplatin were also measured with typically order of magnitude improvements in signal. These and other examples show clearly the benefits that can be obtained in high sensitivity mass spectrometry of biomolecules with the increasing availability of VUV laser sources
Photoion spectroscopy of atoms using coincidence techniques
International Nuclear Information System (INIS)
Hayaishi, Tatsuji
1990-01-01
Interaction of atoms or molecules with photons causes many effects which are often obscured because of many decay paths from the event. To pick up an effect in the mixed-up ones, it is necessary to observe the decay path arising the effect alone. There is a coincidence technique in one of experimental means for the purpose of observing the decay path. In this article, two coincidence measurements are presented; a photoelectron-photoion coincidence technique and a threshold photoelectron-photoion coincidence technique. Furthermore, experimental facts of rare gases atoms obtained by the techniques are reviewed. (author)
Cosmic-Ray Propagation in Turbulent Spiral Magnetic Fields Associated with Young Stellar Objects
Fatuzzo, Marco; Adams, Fred C.
2018-04-01
External cosmic rays impinging upon circumstellar disks associated with young stellar objects provide an important source of ionization, and, as such, play an important role in disk evolution and planet formation. However, these incoming cosmic rays are affected by a variety of physical processes internal to stellar/disk systems, including modulation by turbulent magnetic fields. Globally, these fields naturally provide both a funneling effect, where cosmic rays from larger volumes are focused into the disk region, and a magnetic mirroring effect, where cosmic rays are repelled due to the increasing field strength. This paper considers cosmic-ray propagation in the presence of a turbulent spiral magnetic field, analogous to that produced by the solar wind. The interaction of this wind with the interstellar medium defines a transition radius, analogous to the heliopause, which provides the outer boundary to this problem. We construct a new coordinate system where one coordinate follows the spiral magnetic field lines and consider magnetic perturbations to the field in the perpendicular directions. The presence of magnetic turbulence replaces the mirroring points with a distribution of values and moves the mean location outward. Our results thus help quantify the degree to which cosmic-ray fluxes are reduced in circumstellar disks by the presence of magnetic field structures that are shaped by stellar winds. The new coordinate system constructed herein should also be useful in other astronomical applications.
Laboratory Photoionization Fronts in Nitrogen Gas: A Numerical Feasibility and Parameter Study
Gray, William J.; Keiter, P. A.; Lefevre, H.; Patterson, C. R.; Davis, J. S.; van Der Holst, B.; Powell, K. G.; Drake, R. P.
2018-05-01
Photoionization fronts play a dominant role in many astrophysical situations but remain difficult to achieve in a laboratory experiment. We present the results from a computational parameter study evaluating the feasibility of the photoionization experiment presented in the design paper by Drake et al. in which a photoionization front is generated in a nitrogen medium. The nitrogen gas density and the Planckian radiation temperature of the X-ray source define each simulation. Simulations modeled experiments in which the X-ray flux is generated by a laser-heated gold foil, suitable for experiments using many kJ of laser energy, and experiments in which the flux is generated by a “z-pinch” device, which implodes a cylindrical shell of conducting wires. The models are run using CRASH, our block-adaptive-mesh code for multimaterial radiation hydrodynamics. The radiative transfer model uses multigroup, flux-limited diffusion with 30 radiation groups. In addition, electron heat conduction is modeled using a single-group, flux-limited diffusion. In the theory, a photoionization front can exist only when the ratios of the electron recombination rate to the photoionization rate and the electron-impact ionization rate to the recombination rate lie in certain ranges. These ratios are computed for several ionization states of nitrogen. Photoionization fronts are found to exist for laser-driven models with moderate nitrogen densities (∼1021 cm‑3) and radiation temperatures above 90 eV. For “z-pinch”-driven models, lower nitrogen densities are preferred (<1021 cm‑3). We conclude that the proposed experiments are likely to generate photoionization fronts.
Triggering Excimer Lasers by Photoionization from Corona Discharges
Xiong, Zhongmin; Duffey, Thomas; Brown, Daniel; Kushner, Mark
2009-10-01
High repetition rate ArF (192 nm) excimer lasers are used for photolithography sources in microelectronics fabrication. In highly attaching gas mixtures, preionization is critical to obtaining stable, reproducible glow discharges. Photoionization from a separate corona discharge is one technique for preionization which triggers the subsequent electron avalanche between the main electrodes. Photoionization triggering of an ArF excimer laser sustained in multi-atmosphere Ne/Ar/F2/Xe gas mixtures has been investigated using a 2-dimensional plasma hydrodynamics model including radiation transport. Continuity equations for charged and neutral species, and Poisson's equation are solved coincident with the electron temperature with transport coefficients obtained from solutions of Boltzmann's equation. Photoionizing radiation is produced by a surface discharge which propagates along a corona-bar located adjacent to the discharge electrodes. The consequences of pulse power waveform, corona bar location, capacitance and gas mixture on uniformity, symmetry and gain of the avalanche discharge will be discussed.
Effects of Combined Stellar Feedback on Star Formation in Stellar Clusters
Wall, Joshua Edward; McMillan, Stephen; Pellegrino, Andrew; Mac Low, Mordecai; Klessen, Ralf; Portegies Zwart, Simon
2018-01-01
We present results of hybrid MHD+N-body simulations of star cluster formation and evolution including self consistent feedback from the stars in the form of radiation, winds, and supernovae from all stars more massive than 7 solar masses. The MHD is modeled with the adaptive mesh refinement code FLASH, while the N-body computations are done with a direct algorithm. Radiation is modeled using ray tracing along long characteristics in directions distributed using the HEALPIX algorithm, and causes ionization and momentum deposition, while winds and supernova conserve momentum and energy during injection. Stellar evolution is followed using power-law fits to evolution models in SeBa. We use a gravity bridge within the AMUSE framework to couple the N-body dynamics of the stars to the gas dynamics in FLASH. Feedback from the massive stars alters the structure of young clusters as gas ejection occurs. We diagnose this behavior by distinguishing between fractal distribution and central clustering using a Q parameter computed from the minimum spanning tree of each model cluster. Global effects of feedback in our simulations will also be discussed.
Rotationally resolved flurorescence as a probe of molecular photoionization dynamics
International Nuclear Information System (INIS)
Poliakoff, E.D.; Kakar, S.; Choi, H.C.
1993-01-01
We present rotationally resolved data for N 2 (2σ u -1 ) photoionization in the excitation energy range 19 ≤ hν ≤ 35 eV. These are the first rotationally resolved measurements on the photoion over an extended spectral range above the ionization threshold. The requisite resolution is obtained by measuring rotationally resolved fluorescence from electronically excited photoions created by synchrotron radiation. This technique is useful for studying dynamical features embedded deep in the ionization continua and should supplement laser-based methods that are limited to probing near-threshold phenomena. The present study shows that the outgoing photoelectron can alter the rotational motion of the more massive photoion by exchanging angular momentum and this partitioning of angular momentum depends on the ionization dynamics. Thus, our data directly probe electron-molecule interactions and are sensitive probes of scattering dynamics. We are currently investigating dynamical features such as shape resonances and Cooper minima with rotational resolution for deciphering microscopic aspects of molecular scattering and these efforts will be discussed
Photoionization of subvalence p-subshell in alkali and alkaline-earth atoms
International Nuclear Information System (INIS)
Yagishita, A.; Hayaishi, T.; Itoh, Y.
1986-11-01
Photoionization of alkali and alkaline-earth atoms has been investigated by means of a time-of-flight mass spectrometer combined with monochromatised synchrotron radiation and an atomic beam, in the wavelength region of 350 - 750 A. For alkaline-earth atoms, it has been made clear that a two-step autoionization following an innershell excitation plays an important role for doubly charged ions. For alkali atoms, relative photoionization cross sections have been measured for the first time. Moreover, a tentative assignment of spectral lines for Rb and Cs in the complex spectral region has been attemped based on the photoionization data. (author)
Protonation enhancement by dichloromethane doping in low-pressure photoionization.
Shu, Jinian; Zou, Yao; Xu, Ce; Li, Zhen; Sun, Wanqi; Yang, Bo; Zhang, Haixu; Zhang, Peng; Ma, Pengkun
2016-12-01
Doping has been used to enhance the ionization efficiency of analytes in atmospheric pressure photoionization, which is based on charge exchange. Compounds with excellent ionization efficiencies are usually chosen as dopants. In this paper, we report a new phenomenon observed in low-pressure photoionization: Protonation enhancement by dichloromethane (CH 2 Cl 2 ) doping. CH 2 Cl 2 is not a common dopant due to its high ionization energy (11.33 eV). The low-pressure photoionization source was built using a krypton VUV lamp that emits photons with energies of 10.0 and 10.6 eV and was operated at ~500-1000 Pa. Protonation of water, methanol, ethanol, and acetaldehyde was respectively enhanced by 481.7 ± 122.4, 197.8 ± 18.8, 87.3 ± 7.8, and 93.5 ± 35.5 times after doping 291 ppmv CH 2 Cl 2 , meanwhile CH 2 Cl 2 almost does not generate noticeable ions itself. This phenomenon has not been documented in the literature. A new protonation process involving in ion-pair and H-bond formations was proposed to expound the phenomenon. The observed phenomenon opens a new prospect for the improvement of the detection efficiency of VUV photoionization.
TRACING THE EVOLUTION OF HIGH-REDSHIFT GALAXIES USING STELLAR ABUNDANCES
Energy Technology Data Exchange (ETDEWEB)
Crosby, Brian D.; O’Shea, Brian W. [Department of Physics and Astronomy, Michigan State University, East Lansing, MI 48824 (United States); Beers, Timothy C. [Department of Physics and JINA—Center for the Evolution of the Elements, University of Notre Dame, 225 Nieuwland Science Hall, Notre Dame, IN 46556 (United States); Tumlinson, Jason, E-mail: crosby.bd@gmail.com [Space Telescope Science Institute, 3700 San Martin Drive, Baltimore, MD 21218 (United States)
2016-03-20
This paper presents the first results from a model for chemical evolution that can be applied to N-body cosmological simulations and quantitatively compared to measured stellar abundances from large astronomical surveys. This model convolves the chemical yield sets from a range of stellar nucleosynthesis calculations (including asymptotic giant branch stars, Type Ia and II supernovae, and stellar wind models) with a user-specified stellar initial mass function (IMF) and metallicity to calculate the time-dependent chemical evolution model for a “simple stellar population” (SSP) of uniform metallicity and formation time. These SSP models are combined with a semianalytic model for galaxy formation and evolution that uses merger trees from N-body cosmological simulations to track several α- and iron-peak elements for the stellar and multiphase interstellar medium components of several thousand galaxies in the early (z ≥ 6) universe. The simulated galaxy population is then quantitatively compared to two complementary data sets of abundances in the Milky Way stellar halo and is capable of reproducing many of the observed abundance trends. The observed abundance ratio distributions are best reproduced with a Chabrier IMF, a chemically enriched star formation efficiency of 0.2, and a redshift of reionization of 7. Many abundances are qualitatively well matched by our model, but our model consistently overpredicts the carbon-enhanced fraction of stars at low metallicities, likely owing to incomplete coverage of Population III stellar yields and supernova models and the lack of dust as a component of our model.
Double photoionization of H2: An experimental test of electronic-correlation models in molecules
International Nuclear Information System (INIS)
Dujardin, G.; Besnard, M.J.; Hellner, L.; Malinovitch, Y.
1987-01-01
The double-photoionization cross sections of molecular hydrogen (H 2 ) and molecular deuterium (D 2 ) were measured by using the photoion-photoion coincidence method for photon energies ranging from the threshold energy around 50 eV up to, respectively, 140 and 98 eV. The comparison with the recent ab initio calculations of Le Rouzo [J. Phys. B 19, L677 (1986)] indicates that an important part of the double-photoionization process is accounted for by a rigorous description of the electron-electron interaction in the initial state. As a by-product of this work, it was also concluded that double photoionization of hydrogen can be considered as a vertical process and that Franck-Condon approximations are quite valid to calculate the kinetic energy of the resulting H + +H + fragments
The National Programme of Stellar Physics. Assessment 2011-2014. Prospective 2015-2018
International Nuclear Information System (INIS)
Bontemps, Sylvain; Bouchy, Francois; Charbonnel, Corinne; Chieze, Jean-Pierre; Dessart, Luc; Dintrans, Boris; Dougados, Catherine; Josselin, Eric; Kervella, Pierre; Martins, Fabrice; Michel, Eric; Moraux, Estelle; Recio-Blanco, Alejandra; Ristorcelli, Isabelle; Reyle, Celine; Alecian, Evelyne; Bouchy, Francois; Ciardi, Andrea; Dintrans, Boris; Herpin, Fabrice; Jouve, Laurene; Lebreton, Yveline; Motte, Frederique; Nardetto, Nicolas; Robin, Annie; Royer, Frederic; Samadi, Reza
2015-04-01
After an introduction which outlines the role of stellar physics as a keystone of research in astrophysics, this report proposes a presentation of the operation of the French national programme of stellar physics (PNPS): status and general operation, annual operation, statistics of budget and calls for bids, scientific animation, education, communication, community census, assessment of projects and thesis. It presents an overview of priority research theses between 2011 and 2014, according to their theme: stellar formation and protoplanetary disks, stellar structure and evolutions, origin and impact of magnetism, and atmospheres, winds and mass loss. Transverse theses are also presented the same way for the same period, with the following themes: basic physics, numeric simulations. The last part presents prospectives in terms of events (colloquium), bodies (new scientific council), themes to be studied, operation (interdisciplinarity and interfaces), means, general recommendations, and strengths and weaknesses of the national community
A theoretical study on the photoionization of the valence orbitals of phosphine
Directory of Open Access Journals (Sweden)
Nascimento Edmar M.
2006-01-01
Full Text Available We report a theoretical study on the photoionization of phosphine in the static-exchange level and frozen core approximation, using the method of continued fractions. The main subject of the present study is to investigate in which extent the Hartree-Fock description of the target applied to molecular photoionization is valid. Also, the role played by multichannel coupling is analysed. Our study shows that single-channel Hartree-Fock calculations can provide reliable results except for photon energies near the photoionization threshold.
Photoionization dynamics of excited Ne, Ar, Kr and Xe atoms near threshold
International Nuclear Information System (INIS)
Sukhorukov, V L; Petrov, I D; Schäfer, M; Merkt, F; Ruf, M-W; Hotop, H
2012-01-01
A review of experimental and theoretical studies of the threshold photoionization of the heavier rare-gas atoms is presented, with particular emphasis on the autoionization resonances in the spectral region between the lowest two ionization thresholds 2 P 3/2 and 2 P 1/2 , accessed from the ground or excited states. Observed trends in the positions, widths and shapes of the autoionization resonances depending on the atomic number, the principal quantum number n, the orbital angular momentum quantum number ℓ and further quantum numbers specifying the fine- and hyperfine-structure levels are summarized and discussed in the light of ab initio and multichannel quantum defect theory calculations. The dependence of the photoionization spectra on the initially prepared neutral state are also discussed, including results on the photoionization cross sections and photoelectron angular distributions of polarized excited states. The effects of various approximations in the theoretical treatment of photoionization in these systems are analysed. The very large diversity of observed phenomena and the numerous anomalies in spectral structures associated with the threshold ionization of the rare-gas atoms can be described in terms of a limited set of interactions and dynamical processes. Examples are provided illustrating characteristic aspects of the photoionization, and sets of recommended parameters describing the energy-level structure and photoionization dynamics of the rare-gas atoms are presented which were extracted in a critical analysis of the very large body of experimental and theoretical data available on these systems in the literature. (topical review)
Molecular alignment dependent electron interference in attosecond ultraviolet photoionization
Directory of Open Access Journals (Sweden)
Kai-Jun Yuan
2015-01-01
Full Text Available We present molecular photoionization processes by intense attosecond ultraviolet laser pulses from numerical solutions of time-dependent Schrödinger equations. Simulations preformed on a single electron diatomic H2+ show minima in molecular photoelectron energy spectra resulting from two center interference effects which depend strongly on molecular alignment. We attribute such sensitivity to the spatial orientation asymmetry of the photoionization process from the two nuclei. A similar influence on photoelectron kinetic energies is also presented.
Molecular alignment dependent electron interference in attosecond ultraviolet photoionization
Yuan, Kai-Jun; Bandrauk, André D.
2015-01-01
We present molecular photoionization processes by intense attosecond ultraviolet laser pulses from numerical solutions of time-dependent Schrödinger equations. Simulations preformed on a single electron diatomic H2+ show minima in molecular photoelectron energy spectra resulting from two center interference effects which depend strongly on molecular alignment. We attribute such sensitivity to the spatial orientation asymmetry of the photoionization process from the two nuclei. A similar influence on photoelectron kinetic energies is also presented. PMID:26798785
VUV photoionization cross sections of HO2, H2O2, and H2CO.
Dodson, Leah G; Shen, Linhan; Savee, John D; Eddingsaas, Nathan C; Welz, Oliver; Taatjes, Craig A; Osborn, David L; Sander, Stanley P; Okumura, Mitchio
2015-02-26
The absolute vacuum ultraviolet (VUV) photoionization spectra of the hydroperoxyl radical (HO2), hydrogen peroxide (H2O2), and formaldehyde (H2CO) have been measured from their first ionization thresholds to 12.008 eV. HO2, H2O2, and H2CO were generated from the oxidation of methanol initiated by pulsed-laser-photolysis of Cl2 in a low-pressure slow flow reactor. Reactants, intermediates, and products were detected by time-resolved multiplexed synchrotron photoionization mass spectrometry. Absolute concentrations were obtained from the time-dependent photoion signals by modeling the kinetics of the methanol oxidation chemistry. Photoionization cross sections were determined at several photon energies relative to the cross section of methanol, which was in turn determined relative to that of propene. These measurements were used to place relative photoionization spectra of HO2, H2O2, and H2CO on an absolute scale, resulting in absolute photoionization spectra.
K-SHELL PHOTOIONIZATION OF NICKEL IONS USING R-MATRIX
International Nuclear Information System (INIS)
Witthoeft, M. C.; Bautista, M. A.; GarcIa, J.; Kallman, T. R.; Mendoza, C.; Palmeri, P.; Quinet, P.
2011-01-01
We present R-matrix calculations of photoabsorption and photoionization cross sections across the K edge of the Li-like to Ca-like ion stages of Ni. Level-resolved, Breit-Pauli calculations were performed for the Li-like to Na-like stages. Term-resolved calculations, which include the mass-velocity and Darwin relativistic corrections, were performed for the Mg-like to Ca-like ion stages. This data set is extended up to Fe-like Ni using the distorted wave approximation as implemented by AUTOSTRUCTURE. The R-matrix calculations include the effects of radiative and Auger dampings by means of an optical potential. The damping processes affect the absorption resonances converging to the K thresholds causing them to display symmetric profiles of constant width that smear the otherwise sharp edge at the K-shell photoionization threshold. These data are important for the modeling of features found in photoionized plasmas.
K-Shell Photoionization of Nickel Ions Using R-Matrix
Witthoeft, M. C.; Bautista, M. A.; Garcia, J.; Kallman, T. R.; Mendoza, C.; Palmeri, P.; Quinet, P.
2011-01-01
We present R-matrix calculations of photoabsorption and photoionization cross sections across the K edge of the Li-like to Ca-like ions stages of Ni. Level-resolved, Breit-Pauli calculations were performed for the Li-like to Na-like stages. Term-resolved calculations, which include the mass-velocity and Darwin relativistic corrections, were performed for the Mg-like to Ca-like ion stages. This data set is extended up to Fe-like Ni using the distorted wave approximation as implemented by AUTOSTRUCTURE. The R-matrix calculations include the effects of radiative and Auger dampings by means of an optical potential. The damping processes affect the absorption resonances converging to the K thresholds causing them to display symmetric profiles of constant width that smear the otherwise sharp edge at the K-shell photoionization threshold. These data are important for the modeling of features found in photoionized plasmas.
Photoionization of furan from the ground and excited electronic states.
Ponzi, Aurora; Sapunar, Marin; Angeli, Celestino; Cimiraglia, Renzo; Došlić, Nađa; Decleva, Piero
2016-02-28
Here we present a comparative computational study of the photoionization of furan from the ground and the two lowest-lying excited electronic states. The study aims to assess the quality of the computational methods currently employed for treating bound and continuum states in photoionization. For the ionization from the ground electronic state, we show that the Dyson orbital approach combined with an accurate solution of the continuum one particle wave functions in a multicenter B-spline basis, at the density functional theory (DFT) level, provides cross sections and asymmetry parameters in excellent agreement with experimental data. On the contrary, when the Dyson orbitals approach is combined with the Coulomb and orthogonalized Coulomb treatments of the continuum, the results are qualitatively different. In excited electronic states, three electronic structure methods, TDDFT, ADC(2), and CASSCF, have been used for the computation of the Dyson orbitals, while the continuum was treated at the B-spline/DFT level. We show that photoionization observables are sensitive probes of the nature of the excited states as well as of the quality of excited state wave functions. This paves the way for applications in more complex situations such as time resolved photoionization spectroscopy.
THE DISK WIND IN THE RAPIDLY SPINNING STELLAR-MASS BLACK HOLE 4U 1630–472 OBSERVED WITH NuSTAR
Energy Technology Data Exchange (ETDEWEB)
King, Ashley L.; Miller, Jon M. [Department of Astronomy, University of Michigan, 500 Church Street, Ann Arbor, MI 48109-1042 (United States); Walton, Dominic J.; Fürst, Felix; Harrison, Fiona A. [Cahill Center for Astronomy and Astrophysics, California Institute of Technology, Pasadena, CA 91125 (United States); Barret, Didier [Université de Toulouse, UPS-OMP, IRAP, Toulouse (France); Boggs, Steven E.; Craig, William W.; Krivonos, Roman; Tomsick, John A. [Space Sciences Laboratory, 7 Gauss Way, University of California, Berkeley, CA 94720-7450 (United States); Christensen, Finn E. [DTU Space, National Space Institute, Technical University of Denmark, Elektrovej 327, DK-2800 Lyngby (Denmark); Fabian, Andy C. [Institute of Astronomy, University of Cambridge, Madingley Road, Cambridge CB3 0HA (United Kingdom); Hailey, Charles J.; Mori, Kaya [Columbia Astrophysics Laboratory, Columbia University, New York, NY 10027 (United States); Natalucci, Lorenzo [Istituto Nazionale di Astrofisica, INAF-IAPS, via del Fosso del Cavaliere, I-00133 Roma (Italy); Stern, Daniel [Jet Propulsion Laboratory, California Institute of Technology, 4800 Oak Grove Drive, Mail Stop 169-221, Pasadena, CA 91109 (United States); Zhang, William W., E-mail: ashking@umich.edu [NASA Goddard Space Flight Center, Greenbelt, MD 20771 (United States)
2014-03-20
We present an analysis of a short NuSTAR observation of the stellar-mass black hole and low-mass X-ray binary 4U 1630–472. Reflection from the inner accretion disk is clearly detected for the first time in this source, owing to the sensitivity of NuSTAR. With fits to the reflection spectrum, we find evidence for a rapidly spinning black hole, a{sub ∗}=0.985{sub −0.014}{sup +0.005} (1σ statistical errors). However, archival data show that the source has relatively low radio luminosity. Recently claimed relationships between jet power and black hole spin would predict either a lower spin or a higher peak radio luminosity. We also report the clear detection of an absorption feature at 7.03 ± 0.03 keV, likely signaling a disk wind. If this line arises in dense, moderately ionized gas (log ξ=3.6{sub −0.3}{sup +0.2}) and is dominated by He-like Fe XXV, the wind has a velocity of v/c=0.043{sub −0.007}{sup +0.002} (12900{sub −2100}{sup +600} km s{sup –1}). If the line is instead associated with a more highly ionized gas (log ξ=6.1{sub −0.6}{sup +0.7}), and is dominated by Fe XXVI, evidence of a blueshift is only marginal, after taking systematic errors into account. Our analysis suggests the ionized wind may be launched within 200-1100 Rg, and may be magnetically driven.
HIGH-RESOLUTION X-RAY SPECTROSCOPY REVEALS THE SPECIAL NATURE OF WOLF-RAYET STAR WINDS
Energy Technology Data Exchange (ETDEWEB)
Oskinova, L. M.; Hamann, W.-R. [Institute for Physics and Astronomy, University Potsdam, 14476 Potsdam (Germany); Gayley, K. G. [Department of Physics and Astronomy, University of Iowa, Iowa City, IA 52245 (United States); Huenemoerder, D. P. [Massachusetts Institute of Technology, Kavli Institute for Astrophysics and Space Research, 70 Vassar St., Cambridge, MA 02139 (United States); Ignace, R. [Department of Physics and Astronomy, East Tennessee State University, Johnson City, TN 37663 (United States); Pollock, A. M. T., E-mail: lida@astro.physik.uni-potsdam.de [European Space Agency XMM-Newton Science Operations Centre, European Space Astronomy Centre, Apartado 78, Villanueva de la Canada, 28691 Madrid (Spain)
2012-03-10
We present the first high-resolution X-ray spectrum of a putatively single Wolf-Rayet (WR) star. 400 ks observations of WR 6 by the XMM-Newton telescope resulted in a superb quality high-resolution X-ray spectrum. Spectral analysis reveals that the X-rays originate far out in the stellar wind, more than 30 stellar radii from the photosphere, and thus outside the wind acceleration zone where the line-driving instability (LDI) could create shocks. The X-ray emitting plasma reaches temperatures up to 50 MK and is embedded within the unshocked, 'cool' stellar wind as revealed by characteristic spectral signatures. We detect a fluorescent Fe line at Almost-Equal-To 6.4 keV. The presence of fluorescence is consistent with a two-component medium, where the cool wind is permeated with the hot X-ray emitting plasma. The wind must have a very porous structure to allow the observed amount of X-rays to escape. We find that neither the LDI nor any alternative binary scenario can explain the data. We suggest a scenario where X-rays are produced when the fast wind rams into slow 'sticky clumps' that resist acceleration. Our new data show that the X-rays in single WR star are generated by some special mechanism different from the one operating in the O-star winds.
Technological aspects of the Wega stellarator
International Nuclear Information System (INIS)
Fritsch, R.; Ohlendorf, W.; Pacher, G.W.; Pacher, H.D.; Wegrowe, J.G.; Lipa, M.; CEA Centre d'Etudes Nucleaires de Grenoble, 38
1976-01-01
Wega, an ohmically heated Stellarator at Grenoble for the study of R.F. heating at high power. On the vacuum vessel are mounted helical windings with periods l=2, m=5, designed to produce a rotational transform of 0.3 at a main field of 2.5T. Calculations to simulate the effect of the stray flux of the transformer yokes show that a vertical field variation of the same periodicity as the helical windings (five-fold symmetry) does not affect the magnetic surfaces. Accordingly five transformer yokes are used. To assemble internal R.F. structures, it was required that the two halves of the device be separable, therefore electrically and mechanically distinct. The 14 helical conductors of the 4 windings of each of the device are placed in series by means of end connections magnetically compensated. To facilitate further the separability of the two halves, one of them, weighing 5 tons (vacuum vessel, toroidal field coils, supporting structures) is supported at three points, and can be displaced horizontally by 3m using an air cushion system [fr
International Nuclear Information System (INIS)
Dolmatov, V K; Craven, G T; Keating, D
2010-01-01
Trends in resonances, termed confinement resonances, in photoionization of atoms A in endohedral fullerene anions A-C z- 60 are theoretically studied and exemplified by the photoionization of Ne in Ne-C z- 60 . Remarkably, above a particular nl ionization threshold of Ne in neutral Ne-C 60 (I z=0 nl ), confinement resonances in corresponding partial photoionization cross sections σ nl of Ne in any charged Ne-C z- 60 are not affected by a variation in the charge z of the carbon cage, as a general phenomenon. At lower photon energies, ω z=0 nl , the corresponding photoionization cross sections of charged Ne-C z- 60 (i.e., those with z ≠ 0) develop additional, strong, z-dependent resonances, termed Coulomb confinement resonances, as a general occurrence. Furthermore, near the innermost 1s ionization threshold, the 2p photoionization cross section σ 2p of the outermost 2p subshell of thus confined Ne is found to inherit the confinement resonance structure of the 1s photoionization spectrum, via interchannel coupling. As a result, new confinement resonances emerge in the 2p photoionization cross section of the confined Ne atom at photoelectron energies which exceed the 2p threshold by about a thousand eV, i.e., far above where conventional wisdom said they would exist. Thus, the general possibility for confinement resonances to resurrect in photoionization spectra of encapsulated atoms far above thresholds is revealed, as an interesting novel general phenomenon.
Photoionization sensors for non-invasive medical diagnostics
Mustafaev, Aleksandr; Rastvorova, Iuliia; Khobnya, Kristina; Podenko, Sofia
2016-09-01
The analysis of biomarkers can help to identify the significant number of diseases: lung cancer, tuberculosis, diabetes, high levels of stress, psychosomatic disorders etc. To implement continuous monitoring of the state of human health, compact VUV photoionization detector with current-voltage measurement is designed by Saint-Petersburg Mining University Plasma Research Group. This sensor is based on the patented method of stabilization of electric parameters - CES (Collisional Electron Spectroscopy). During the operation at atmospheric pressure VUV photoionization sensor measures the energy of electrons, produced in the ionization with the resonance photons, whose wavelength situated in the vacuum ultraviolet (VUV). A special software was developed to obtain the second-order derivative of the I-U characteristics, taken by the VUV sensor, to construct the energy spectra of the characteristic electrons. VUV photoionization detector has an unique set of parameters: small size (10*10*1 mm), low cost, wide range of recognizable molecules, as well as accuracy, sufficient for using this instrument for the medical purposes. This device can be used for non-invasive medical diagnostics without compromising the quality of life, for control of environment and human life. Work supported by Foundation for Assistance to Small Innovative Enterprises in Science and Technology.
Photoionization cross sections and Auger rates calculated by many-body perturbation theory
International Nuclear Information System (INIS)
Kelly, H.P.
1976-01-01
Methods for applying the many body perturbation theory to atomic calculations are discussed with particular emphasis on calculation of photoionization cross sections and Auger rates. Topics covered include: Rayleigh--Schroedinger theory; many body perturbation theory; calculations of photoionization cross sections; and Auger rates
Photoionization mass spectrometry of UF6
International Nuclear Information System (INIS)
Berkowitz, J.
1979-01-01
The photoionization mass spectrum of 238 UF 6 was obtained. At 600 A = 20.66 eV, the relative ionic abundances were as follows: UF 6 + , 1.4; UF 5 + , 100; UF + , 17; UF 3 + , approx. 0.7; UF 2 + , very weak; UF + , very weak; U + , essentially zero. The adiabatic ionization potential for UF 6 was 13.897 +- 0.005 eV. The production of UF 5 + begins at approx. 887 A = 13.98 eV, at which energy the UF 6 + partial cross section abruptly declines and then levels off. This behavior suggests the vague possibility of an isotope effect. The UF 4 + signal begins at approx. 725 A = 17.10 eV, at which energy the UF 5 + signal reaches a plateau value. The UF 5 + photoionization yield curve displays some autoionization structure from its threshold to approx. 750 A
Photoionization of atoms. Progress report, 1 April 1979-30 March 1980
International Nuclear Information System (INIS)
Samson, J.A.R.; Starace, A.F.
1979-12-01
A strong 304 A fluorescent signal from He + (n = 2) has been observed as a function of incident photon wavelength; strong autoionizing structure arising from 3n + states are seen in the spectrum. Measurements of the ratio of photoproduced Ne + ions to Ne 2+ ions indicate that further calibration of detector response is required. The dissociative photoionization of O 2 has been measured successfully as a necessary preliminary to measuring the photoionization cross section of atomic oxygen. The experimental apparatus has been built to measure the photoelectron angular distribution of atomic cesium. In order to measure rare gas photoionization cross sections to +-1% accuracy, a new gas tight window has been developed and second order lines in the laboratory light sources have been classified. A new random phase approximation (RPA) for the theoretical calculation of open- or closed-shell atom photoionization cross sections has been developed; the close-coupling approximation and the closed-shell atom RPA of Chang and Fano are limiting cases of a new set of coupled differential equations. The Rydberg energy spectrum and oscillator strengths of atomic hydrogen have been calculated for magnetic fields of order 10 5 Gauss using a basis of oblate spheroidal angle functions. Below N approx. = 12 an adiabatic approximation is excellent. Above n approx. = 12 non-adiabatic coupling terms rapidly become important, and the perturbed energy levels for n greater than or equal to 16 cross, indicating quasi-conserved dynamical symmetries. A previous calculation of the cesium 6s → epsilon p photoionization cross section has been extended to include interchannel coupling to the 5p → epsilon d photoionization channels; above the near threshold cross section minimum, the cross section is dominated by 5p → 5d resonance transitions
Combined corona discharge and UV photoionization source for ion mobility spectrometry.
Bahrami, Hamed; Tabrizchi, Mahmoud
2012-08-15
An ion mobility spectrometer is described which is equipped with two non-radioactive ion sources, namely an atmospheric pressure photoionization and a corona discharge ionization source. The two sources cannot only run individually but are additionally capable of operating simultaneously. For photoionization, a UV lamp was mounted parallel to the axis of the ion mobility cell. The corona discharge electrode was mounted perpendicular to the UV radiation. The total ion current from the photoionization source was verified as a function of lamp current, sample flow rate, and drift field. Simultaneous operation of the two ionization sources was investigated by recording ion mobility spectra of selected samples. The design allows one to observe peaks from either the corona discharge or photoionization individually or simultaneously. This makes it possible to accurately compare peaks in the ion mobility spectra from each individual source. Finally, the instrument's capability for discriminating two peaks appearing in approximately identical drift times using each individual ionization source is demonstrated. Copyright © 2012 Elsevier B.V. All rights reserved.
Xu, Jing; Sang, Pengpeng; Zhao, Lianming; Guo, Wenyue; Qi, Fei; Xing, Wei; Yan, Zifeng
The photoionization and fragmentation of octadecane were investigated with infrared laser desorption/tunable synchrotron vacuum ultraviolet (VUV) photoionization mass spectrometry (IRLD/VUV PIMS) and theoretical calculations. Mass spectra of octadecane were measured at various photon energies. The fragment ions were gradually detected with the increase of photon energy. The main fragment ions were assigned to radical ions (C n H 2 n +1 + , n = 4-11) and alkene ions (C n H 2 n + , n = 5-10). The ionization energy of the precursor and appearance energy of ionic fragments were obtained by measuring the photoionization efficiency spectrum. Possible formation pathways of the fragment ions were discussed with the help of density functional theory calculations.
Photoionization microscopy of Rydberg hydrogen atom in a non-uniform electrical field
International Nuclear Information System (INIS)
Cheng Shao-Hao; Wang De-Hua; Chen Zhao-Hang; Chen Qiang
2016-01-01
In this paper, we investigate the photoionization microscopy of the Rydberg hydrogen atom in a gradient electric field for the first time. The observed oscillatory patterns in the photoionization microscopy are explained within the framework of the semiclassical theory, which can be considered as a manifestation of interference between various electron trajectories arriving at a given point on the detector plane. In contrast with the photoionization microscopy in the uniform electric field, the trajectories of the ionized electron in the gradient electric field will become chaotic. An infinite set of different electron trajectories can arrive at a given point on the detector plane, which makes the interference pattern of the electron probability density distribution extremely complicated. Our calculation results suggest that the oscillatory pattern in the electron probability density distribution depends sensitively on the electric field gradient, the scaled energy and the position of the detector plane. Through our research, we predict that the interference pattern in the electron probability density distribution can be observed in an actual photoionization microscopy experiment once the external electric field strength and the position of the electron detector plane are reasonable. This study provides some references for the future experimental research on the photoionization microscopy of the Rydberg atom in the non-uniform external fields. (paper)
Photoionization mass spectrometric studies of selected compounds in a molecular beam
Energy Technology Data Exchange (ETDEWEB)
Trott, W.M.
1979-03-01
Photoionization efficiency curves have been measured at moderate to high resolution for several species produced in supersonic molecular beams of acetone, acetone-d/sub 6/ and CS/sub 2/. The molecular beam photoionization mass spectrometer which has been assembled for this work is described. The performance of this instrument has been characterized by a number of experiments and calculations.
Photoionization mass spectrometric studies of selected compounds in a molecular beam
International Nuclear Information System (INIS)
Trott, W.M.
1979-03-01
Photoionization efficiency curves have been measured at moderate to high resolution for several species produced in supersonic molecular beams of acetone, acetone-d 6 and CS 2 . The molecular beam photoionization mass spectrometer which has been assembled for this work is described. The performance of this instrument has been characterized by a number of experiments and calculations
International Nuclear Information System (INIS)
Seno, Koichiro; Ishioka, Toshio; Harata, Akira; Hatano, Yoshihiko
2002-01-01
Photoionization spectroscopy using synchrotron radiation as a photon source was applied to the aqueous solution surfaces of rhodamine B (RhB), rhodamine 6G (Rh6G), and rhodamine 101 (Rh101) with their concentration of 0-100 μmol dm -3 . Synchrotron radiation was irradiated upon the solution surface between two electrodes in the photon energy range of 4-7 eV, and photoionization current was measured by a pico-ammeter. The photocurrent for each of the rhodamine aqueous solution surface showed an increase with the photon energy above a threshold photon energy. The photoionization threshold of RhB at the aqueous solution surface was 5.6 eV, which was smaller than that in the gas phase. The intensity of photoionization current of Rh6G was smaller than that of RhB or Rh101. Photoionization processes and the state of Rhodamine dye molecules at the aqueous solution surface were discussed in connection with results of surface tension measurements. (author)
Emission-line widths and stellar-wind flows in T Tauri stars
International Nuclear Information System (INIS)
Sa, C.; Lago, M.T.V.T.
1986-01-01
Spectra are reported of T Tauri stars taken with the IPCS on the Isaac Newton Telescope at the Observatorio del Roque de los Muchachos at a dispersion of l7 A mm -1 . These were taken in order to determine emission-line widths and hence flow velocities in the winds of these stars following the successful modelling of the wind from RU Lupi using such data. Line widths in RW Aur suggest a similar pattern to the wind flow as in RU Lupi with velocities rising in the inner chromosphere of the star and then entering a 'ballistic' zone. The wind from DFTau is also similar but velocities are generally much lower and the lines sharper. (author)
Photoionization studies of atoms and molecules using synchrotron radiation
International Nuclear Information System (INIS)
Lindle, D.W.
1988-01-01
Photoionization studies of free atoms and molecules have undergone considerable development in the past decade, in large part due to the use of synchrotron radiation. The tunability of synchrotron radiation has permitted the study of photoionization processes near valence-and core-level ionization thresholds for atoms and molecules throught the Periodic Table. A general illustration of these types of study will be presented, with emphasis on a few of the more promising new directions in atomic and molecular physics being pursued with synchrotron radiation. (author) [pt
Photodissociation of anisole and absolute photoionization cross-section of the phenoxy radical.
Xu, Hong; Pratt, S T
2013-11-21
We have studied the photodissociation dynamics of anisole (C6H5OCH3) at 193 nm and determined the absolute photoionization cross-section of the phenoxy radical at 118.2 nm (10.486 eV) relative to the known cross-section of the methyl radical. Even at this energy, there is extensive fragmentation of the phenoxy radical upon photoionization, which is attributed to ionizing transitions that populate low-lying excited electronic states of the cation. For phenoxy radicals with less than ∼1 eV of internal energy, we find a cross-section for the production of the phenoxy cation of 14.8 ± 3.8 Mb. For radicals with higher internal energy, dissociative ionization is the dominant process, and for internal energies of ∼2.7-3.7 eV, we find a total cross-section (photoionization plus dissociative ionization) of 22.3 ± 4.1 Mb. The results are discussed relative to the recently reported photoionization cross-section of phenol.
Dissociative photoionization of quinoline and isoquinoline
Bouwman, J.; Sztáray, B.; Oomens, J.; Hemberger, P.; Bodi, A.
2015-01-01
Two nitrogen-containing polycyclic aromatic hydrocarbon isomers of C9H7N composition, quinoline, and isoquinoline have been studied by imaging photoelectron photoion coincidence spectroscopy at the VUV beamline of the Swiss Light Source. High resolution threshold photoelectron spectra have been
Photoionization Modeling and the K Lines of Iron
Kallman, T. R.; Palmeri, P.; Bautista, M. A.; Mendoza, C.; Krolik, J. H.
2004-01-01
We calculate the efficiency of iron K line emission and iron K absorption in photoionized models using a new set of atomic data. These data are more comprehensive than those previously applied to the modeling of iron K lines from photoionized gases, and allow us to systematically examine the behavior of the properties of line emission and absorption as a function of the ionization parameter, density and column density of model constant density clouds. We show that, for example, the net fluorescence yield for the highly charged ions is sensitive to the level population distribution produced by photoionization, and these yields are generally smaller than those predicted assuming the population is according to statistical weight. We demonstrate that the effects of the many strongly damped resonances below the K ionization thresholds conspire to smear the edge, thereby potentially affecting the astrophysical interpretation of absorption features in the 7-9 keV energy band. We show that the centroid of the ensemble of K(alpha) lines, the K(beta) energy, and the ratio of the K(alpha(sub 1)) to K(alpha(sub 2)) components are all diagnostics of the ionization parameter of our model slabs.
International Nuclear Information System (INIS)
Correa, J.D.; Duque, C.A.; Porras-Montenegro, N.
2004-01-01
Full text: Using a variational procedure for a hydrogenic donor-impurity we have calculated the photoionization cross-section in spherical GaAs quantum dots. We discuss the dependence on the photoionization cross-section for hydrogenic donor impurity in in nite and nite barrier quantum dots as a function of the size of the dot, impurity position, polarization of the photon, applied hydrostatic pressure, and normalized photon energy. For the nite case, calculations for the pressure effects are both in direct and indirect GaAsAl gap regime. We have considered the different transition rules that depend of the impurity position and photon polarization. Calculations are presented for impurity on-center, and o -center in the spherical quantum dots. We found that the photoionization cross-section increases with the applied hydrostatic pressure both for on-center and o - center impurities. The photoionization cross-section increases or decreases depending of the impurity position, photon polarization, and radius of dots. Also we have showed that the photoionization cross-section decreases as the normalized photon energy increases. The results we have obtained show that the photoionization cross- section is strongly a effected by the quantum dot size, and the position of the impurity. The measurement of photoionization in such systems would be of great interest in understanding the optical properties of carriers in quantum dots. (author)
Coil development for the quasi-poloidal stellarator project
International Nuclear Information System (INIS)
Nelson, B.E.; Berry, L.A.; Cole, M.J.; Fogarty, P.J.; Freudenberg, K.; Hirshman, S.P.; Lyon, J.F.; Spong, D.A.; Strickler, D.J.; Williamson, D.; Benson, R.D.; Lumsdaine, A.; Madhukar, M.; Parang, M.; Shannon, T.; Dahlgren, F.; Heitzenroeder, P.; Neilson, G.H.; Goranson, P.; Hargrove, T.; Jones, G.; Lovett, G.
2005-01-01
The Quasi-Poloidal Stellarator (QPS), currently in the R and D and prototyping stage, is a low-aspect-ratio (R/a ≥ 2.3), compact stellarator experiment with a non-axisymmetric, near- poloidally-symmetric magnetic field. The QPS design parameters are = 0.95 m, = 0.3-0.4 m, B = 1 T, and a 1.5-s pulse length with 3-5 MW of ECH and ICRF heating power. The most challenging component to design and fabricate is the set of 20 nonplanar modular coils located inside the QPS vacuum tank. There are five distinct coil winding shapes, but only three types of winding forms are needed because each supports two distinct windings and both windings on the most complex coil form are the same shape. The stainless steel winding forms are machined to the required high tolerance and stranded copper cable conductor is wound on the winding forms to the highly precise shape required (to an accuracy of less than 1 mm). The windings are enclosed in a welded, stainless steel cover with stiffeners for compatibility with the QPS vacuum requirements, and the cans are then vacuum pressure impregnated with cynate ester resin to form the finished coil winding pack. Computer modeling and experimental measurements of the welding process indicate that distortion and thermal stress should be acceptable. A prototype coil using the most complex of the three winding forms is being fabricated. The coil winding form has been cast and is being machined to the required tolerance prior to winding with conductor. The machined modular coil forms will be shipped to the winding facility mounted on carts, which provide a work platform for preparing, winding, welding, and potting of the coils. The carts allow rotating the coils for optimum positioning during winding and fabrication. An overhead fixture allows supporting the spools of conductor and feeding the conductor in the correct orientation, groupings, and tensioning. An R and D program is underway that includes extensive conductor characterization and testing
Time-dependent Cooling in Photoionized Plasma
Energy Technology Data Exchange (ETDEWEB)
Gnat, Orly, E-mail: orlyg@phys.huji.ac.il [Racah Institute of Physics, The Hebrew University, Jerusalem 91904 (Israel)
2017-02-01
I explore the thermal evolution and ionization states in gas cooling from an initially hot state in the presence of external photoionizing radiation. I compute the equilibrium and nonequilibrium cooling efficiencies, heating rates, and ion fractions for low-density gas cooling while exposed to the ionizing metagalactic background radiation at various redshifts ( z = 0 − 3), for a range of temperatures (10{sup 8}–10{sup 4} K), densities (10{sup −7}–10{sup 3} cm{sup −3}), and metallicities (10{sup −3}–2 times solar). The results indicate the existence of a threshold ionization parameter, above which the cooling efficiencies are very close to those in photoionization equilibrium (so that departures from equilibrium may be neglected), and below which the cooling efficiencies resemble those in collisional time-dependent gas cooling with no external radiation (and are thus independent of density).
PHOTOIONIZATION MODELS FOR THE SEMI-FORBIDDEN C iii] 1909 EMISSION IN STAR-FORMING GALAXIES
Energy Technology Data Exchange (ETDEWEB)
Jaskot, A. E. [Department of Astronomy, Smith College, Northampton, MA 01063 (United States); Ravindranath, S. [Space Telescope Science Institute, Baltimore, MD 21218 (United States)
2016-12-20
The increasing neutrality of the intergalactic medium at z > 6 suppresses Ly α emission, and spectroscopic confirmation of galaxy redshifts requires the detection of alternative ultraviolet lines. The strong [C iii] λ 1907+C iii] λ 1909 doublet frequently observed in low-metallicity, actively star-forming galaxies is a promising emission feature. We present CLOUDY photoionization model predictions for C iii] equivalent widths (EWs) and line ratios as a function of starburst age, metallicity, and ionization parameter. Our models include a range of C/O abundances, dust content, and gas density. We also examine the effects of varying the nebular geometry and optical depth. Only the stellar models that incorporate binary interaction effects reproduce the highest observed C iii] EWs. The spectral energy distributions from the binary stellar population models also generate observable C iii] over a longer timescale relative to single-star models. We show that diagnostics using C iii] and nebular He ii λ 1640 can separate star-forming regions from shock-ionized gas. We also find that density-bounded systems should exhibit weaker C iii] EWs at a given ionization parameter, and C iii] EWs could, therefore, select candidate Lyman continuum-leaking systems. In almost all models, C iii] is the next strongest line at <2700 Å after Ly α , and C iii] reaches detectable levels for a wide range of conditions at low metallicity. C iii] may therefore serve as an important diagnostic for characterizing galaxies at z > 6.
PHOTOIONIZATION MODELS FOR THE SEMI-FORBIDDEN C iii] 1909 EMISSION IN STAR-FORMING GALAXIES
International Nuclear Information System (INIS)
Jaskot, A. E.; Ravindranath, S.
2016-01-01
The increasing neutrality of the intergalactic medium at z > 6 suppresses Ly α emission, and spectroscopic confirmation of galaxy redshifts requires the detection of alternative ultraviolet lines. The strong [C iii] λ 1907+C iii] λ 1909 doublet frequently observed in low-metallicity, actively star-forming galaxies is a promising emission feature. We present CLOUDY photoionization model predictions for C iii] equivalent widths (EWs) and line ratios as a function of starburst age, metallicity, and ionization parameter. Our models include a range of C/O abundances, dust content, and gas density. We also examine the effects of varying the nebular geometry and optical depth. Only the stellar models that incorporate binary interaction effects reproduce the highest observed C iii] EWs. The spectral energy distributions from the binary stellar population models also generate observable C iii] over a longer timescale relative to single-star models. We show that diagnostics using C iii] and nebular He ii λ 1640 can separate star-forming regions from shock-ionized gas. We also find that density-bounded systems should exhibit weaker C iii] EWs at a given ionization parameter, and C iii] EWs could, therefore, select candidate Lyman continuum-leaking systems. In almost all models, C iii] is the next strongest line at <2700 Å after Ly α , and C iii] reaches detectable levels for a wide range of conditions at low metallicity. C iii] may therefore serve as an important diagnostic for characterizing galaxies at z > 6.
Ion-impact secondary emission in negative corona with photoionization
Directory of Open Access Journals (Sweden)
B. X. Lu
2017-03-01
Full Text Available A corona discharge measurement system and simulation model are presented to investigate the effects of photoionization and ion-impact secondary emission process in negative corona discharge. The simulation results obtained is shown good agreement with experimental observations. Distribution of electron density along the symmetry axis at three critical moments is shown and the role of photoionization in negative corona discharge is clearly explained. Moreover, the current pulses are also presented under different secondary emission coefficients and the effect of the secondary emission coefficient is discussed.
Solvent jet desorption capillary photoionization-mass spectrometry.
Haapala, Markus; Teppo, Jaakko; Ollikainen, Elisa; Kiiski, Iiro; Vaikkinen, Anu; Kauppila, Tiina J; Kostiainen, Risto
2015-03-17
A new ambient mass spectrometry method, solvent jet desorption capillary photoionization (DCPI), is described. The method uses a solvent jet generated by a coaxial nebulizer operated at ambient conditions with nitrogen as nebulizer gas. The solvent jet is directed onto a sample surface, from which analytes are extracted into the solvent and ejected from the surface in secondary droplets formed in collisions between the jet and the sample surface. The secondary droplets are directed into the heated capillary photoionization (CPI) device, where the droplets are vaporized and the gaseous analytes are ionized by 10 eV photons generated by a vacuum ultraviolet (VUV) krypton discharge lamp. As the CPI device is directly connected to the extended capillary inlet of the MS, high ion transfer efficiency to the vacuum of MS is achieved. The solvent jet DCPI provides several advantages: high sensitivity for nonpolar and polar compounds with limit of detection down to low fmol levels, capability of analyzing small and large molecules, and good spatial resolution (250 μm). Two ionization mechanisms are involved in DCPI: atmospheric pressure photoionization, capable of ionizing polar and nonpolar compounds, and solvent assisted inlet ionization capable of ionizing larger molecules like peptides. The feasibility of DCPI was successfully tested in the analysis of polar and nonpolar compounds in sage leaves and chili pepper.
Ionic fragmentation following core-level photoionization of Sn(CH3)4 by soft X-rays
International Nuclear Information System (INIS)
Ueda, Kiyoshi; Shigemasa, Eiji; Sato, Yukinori; Yagishita, Akira; Hayaishi, Tatsuji
1990-01-01
Ionic fragmentation following the photoionization of Sn(CH 3 ) 4 (TMT) has been studied in the photon energy range of 60-600 eV using synchrotron radiation and time-of-flight mass spectrometry. Each of the Sn:4d, 4p, 3d and C:1s photoionization leads to a type of ionic fragmentation that is characteristic of each ionized core. The Sn:4d photoionization above 60 eV predominantly produces the doubly-charged TMT which dissociates into two singly-charged ions and some neutral fragments. The ions produced in this pathway are CH 3 + , C 2 H 3 + , C 2 H 5 + , SnCH m + and/or Sn + . The Sn:4p photoionization produces the triply-charged TMT and enhances the production of H + , CHsub(m' + ) (m' = 0-3) and Sn + significantly. The Sn:3d photoionization produces multiply-charged TMT whose charges are 3-5 and enhances the production of H + , CHsub(m' + ) (m' = 0-2) and Sn + significantly. The C:1s photoionization produces doubly-charged TMT via the KVV Auger transition and enhances the production of CH 3 + , C 2 H 3 + , SnCH m + and/or Sn + . (orig.)
Resonances in electron-molecule scattering and photoionization
International Nuclear Information System (INIS)
Schneider, B.I.; Collins, L.A.
1984-05-01
The development of reliable theoretical models for calculating the decay of quasi-stationary states of molecular systems has become an important endeavor for theoretical chemists. The understanding and analysis of a wide variety of physical and chemical phenomena depend on a knowledge of the behavior of these states in both collisional and photoionization problems. In this article we describe the theory and calculation of these cross sections using our Linear Algebraic/Optical Potential method. The theory makes optimal use of the numerical methods developed to solve large sets of coupled integral equations and the bound state techniques used by quantum chemists. Calculations are presented for a representative class of diatomic and triatomic molecules at varying levels of sophistication and for collisional and photoionization cross sections. 48 references, 11 figures
A non-invasive online photoionization spectrometer for FLASH2
Energy Technology Data Exchange (ETDEWEB)
Braune, Markus, E-mail: markus.braune@desy.de [Deutsches Elektronen-Synchrotron DESY, Notkestrasse 85, 22607 Hamburg (Germany); Brenner, Günter [Paul Scherrer Institut, 5232 Villigen PSI (Switzerland); Dziarzhytski, Siarhei [Deutsches Elektronen-Synchrotron DESY, Notkestrasse 85, 22607 Hamburg (Germany); Juranić, Pavle [Paul Scherrer Institut, 5232 Villigen PSI (Switzerland); Sorokin, Andrey; Tiedtke, Kai [Deutsches Elektronen-Synchrotron DESY, Notkestrasse 85, 22607 Hamburg (Germany)
2016-01-01
A description of the design of an instrument for FEL wavelength monitoring based on photoionization of rare gases is given, as well as a report on calibration and characterization studies. The stochastic nature of the self-amplified spontaneous emission (SASE) process of free-electron lasers (FELs) effects pulse-to-pulse fluctuations of the radiation properties, such as the photon energy, which are determinative for processes of photon–matter interactions. Hence, SASE FEL sources pose a great challenge for scientific investigations, since experimenters need to obtain precise real-time feedback of these properties for each individual photon bunch for interpretation of the experimental data. Furthermore, any device developed to deliver the according information should not significantly interfere with or degrade the FEL beam. Regarding the spectral properties, a device for online monitoring of FEL wavelengths has been developed for FLASH2, which is based on photoionization of gaseous targets and the measurements of the corresponding electron and ion time-of-flight spectra. This paper presents experimental studies and cross-calibration measurements demonstrating the viability of this online photoionization spectrometer.
High Energy Emissions from Young Stellar Objects A. C. Das1 ...
Indian Academy of Sciences (India)
... for the generation of emissions from a YSO on the basis of a simple interaction between the ... important role in generating intense radiation, bipolar flows, stellar winds and many ... Even in the case of a non-rotating compact object, the motion .... The change in energy of the particle due to this electric field is given by. 〈1.
Atomic kinetics of a neon photoionized plasma experiment at Z
Mayes, Daniel C.; Mancini, Roberto; Bailey, James E.; Loisel, Guillaume; Rochau, Gregory; ZAPP Collaboration
2018-06-01
We discuss an experimental effort to study the atomic kinetics in astrophysically relevant photoionized plasmas via K-shell line absorption spectroscopy. The experiment employs the intense x-ray flux emitted at the collapse of a Z-pinch to heat and backlight a photoionized plasma contained within a cm-scale gas cell placed at a variable distance from the Z-pinch and filled with neon gas pressures in the range from 3.5 to 30 Torr. The experimental platform affords an order of magnitude range in the ionization parameter characterizing the photoionized plasma at the peak of the x-ray drive from about 5 to 80 erg*cm/s. Thus, the experiment allows for the study of trends in ionization distribution as a function of the ionization parameter. An x-ray crystal spectrometer capable of time-integrated and/or time-gated configurations is used to collect absorption spectra. The spectra show line absorption by several ionization stages of neon, including Be-, Li-, He-, and H-like ions. Analysis of these spectra yields ion areal densities and charge state distributions, which can be compared with simulation results from atomic kinetics codes. In addition, the electron temperature is extracted from level population ratios of nearby energy levels in Li- and Be-like ions, which can be used to test heating models of photoionized plasmas.
Attosecond-resolved photoionization of chiral molecules.
Beaulieu, S; Comby, A; Clergerie, A; Caillat, J; Descamps, D; Dudovich, N; Fabre, B; Géneaux, R; Légaré, F; Petit, S; Pons, B; Porat, G; Ruchon, T; Taïeb, R; Blanchet, V; Mairesse, Y
2017-12-08
Chiral light-matter interactions have been investigated for two centuries, leading to the discovery of many chiroptical processes used for discrimination of enantiomers. Whereas most chiroptical effects result from a response of bound electrons, photoionization can produce much stronger chiral signals that manifest as asymmetries in the angular distribution of the photoelectrons along the light-propagation axis. We implemented self-referenced attosecond photoelectron interferometry to measure the temporal profile of the forward and backward electron wave packets emitted upon photoionization of camphor by circularly polarized laser pulses. We measured a delay between electrons ejected forward and backward, which depends on the ejection angle and reaches 24 attoseconds. The asymmetric temporal shape of electron wave packets emitted through an autoionizing state further reveals the chiral character of strongly correlated electronic dynamics. Copyright © 2017 The Authors, some rights reserved; exclusive licensee American Association for the Advancement of Science. No claim to original U.S. Government Works.
Modular coil design developments for the National Compact Stellarator Experiment (NCSX)
International Nuclear Information System (INIS)
Williamson, D.; Brooks, A.; Brown, T.; Chrzanowski, J.; Cole, M.; Fan, H.-M.; Freudenberg, K.; Fogarty, P.; Hargrove, T.; Heitzenroeder, P.; Lovett, G.; Miller, P.; Myatt, R.; Nelson, B.; Reiersen, W.; Strickler, D.
2005-01-01
The National Compact Stellarator Experiment (NCSX) is a quasi-axisymmetric facility that combines the high beta and good confinement features of an advanced tokamak with the low current, disruption-free characteristics of a stellarator. The experiment is based on a three field-period plasma configuration with an average major radius of 1.4 m, a minor radius of 0.3 m, and a toroidal magnetic field on axis of up to 2 T. The modular coils are one set in a complex assembly of four coil systems that surround the highly shaped plasma. There are six, each of three coil types in the assembly for a total of 18 modular coils. The coils are constructed by winding copper cable onto a cast stainless steel winding form that has been machined to high accuracy, so that the current center of the winding pack is within ±1.5 mm of its theoretical position. The modular coils operate at a temperature of 80 K and are subjected to rapid heating and stress during a pulse. At this time, the project has completed construction of several prototype components which validate the fabrication and inspection processes that are planned for the production coils. In addition, some advanced techniques for error-field compensation and assembly simulation using computer-aided design (CAD) have been developed
International Nuclear Information System (INIS)
Masuoka, T.; Nakamura, E.
1993-01-01
Single-, double-, and triple-photoionization processes of carbon monoxide (CO) have been studied in the photon-energy region of 37--100 eV by use of time-of-flight mass spectrometry and a photoion-photoion-coincidence method together with synchrotron radiation. The single-, double-, and triple-photoionization cross sections of CO are determined. Ion branching ratios and the partial cross sections for the individual ions respectively produced from the precursors CO + and CO 2+ are determined separately at excitation energies where the molecular and dissociative single- and double-photoionization processes compete. The threshold for the molecular double photoionization was found to be 41.3±0.2 eV. Furthermore, in single photoionization, the production of CO + is dominant whereas with double photoionization dissociation becomes dominant
Strong electron correlation in photoionization of spin-orbit doublets
International Nuclear Information System (INIS)
Amusia, M.Ya.; Chernysheva, L.V.; Manson, S.T.; Msezane, A.M.; Radojevic, V.
2002-01-01
A new and explicitly many-body aspect of the 'leveraging' of the spin-orbit interaction is demonstrated, spin-orbit activated interchannel coupling, which can significantly alter the photoionization cross section of a spin-orbit doublet. As an example, it is demonstrated via a modified version of the spin-polarized random phase approximation with exchange, that a recently observed unexplained structure in the Xe 3d 5/2 photoionization cross section [A. Kivimaeki et al., Phys. Rev. A 63, 012716 (2000)] is entirely due to this effect. Similar features are predicted for Cs 3d 5/2 and Ba 3d 5/2
Higher-order processes in x-ray photoionization of atoms
International Nuclear Information System (INIS)
Kanter, E. P.; Dunford, R. W.; Krassig, B.; Southworth, S. H.; Young, L.
2006-01-01
There are several fourth-generation X-ray light source projects now underway around the world and it is anticipated that by the end of the decade, one or more of these X-ray free-electron lasers will be operational. In this contribution, we describe recent measurements and future plans to study both multielectron and multiphoton atomic photoionization. Although such higher-order processes are rare with present third-generation sources, they will be commonplace in experimental work with the new sources. The topics we discuss here are double K-shell ionization and two-photon X-ray photoionization
International Nuclear Information System (INIS)
Wuilleumier, F.J.
1984-01-01
The status of experiments in photoionization of atoms in excited states is reviewed, with emphasis given to synchrotron and laser photon sources. A technique for exciting the photoionization spectrum of Na atoms using the flux emitted from the bending magnetic of a storage ring is discussed in detail. Some problems in interpreting photoionization spectrum of Ba in the excited state, due to the presence of higher orders are considered. A design approach for a positron storage ring to produce coherent radiation in the VUV is described. It is shown that combined use of a CW dye laser and the positron storage ring will allow new progress to be made in photoionization studies of excited atoms. Some of the experiments to be carried out using the positron storage ring include: measurements of collisional ionization in rare earth metal atoms of low atomic density; photoionization measurements at lower laser powers, leading to an extension of the CW tunability range; and photoionization studies of multiply charged positive ions. 21 references
The photoionization of atomic Eu in the vicinity of its giant resonance
International Nuclear Information System (INIS)
Amusia, M.Ya.
1989-01-01
It is demonstrated that the partial photoionization cross sections of outer subshells of atomic Eu in the giant resonance region are determined by the action of the 4d-electron excitations. The cross section for photoionization of the semifilled 4f 7 subshell is also entirely dominated by the interaction with 4d 10 electrons. (orig.)
Application of a VMI spectrometer to near-threshold photoionization with synchrotron radiation
International Nuclear Information System (INIS)
O'Keeffe, P; Bolognesi, P; Ovcharenko, E; Avaldi, L; Mihelic, A; Richter, R; Moise, A; King, G C
2011-01-01
A new developed velocity map imaging spectrometer has been used to study the photoionization of atoms near threshold. The application of the spectrometer to the measurement of the angular distributions of the photoelectrons emitted in the photoionization of the Ne 2p 3/2 state between the 2p spin orbit thresholds and of polarised Ne atoms are presented.
Absolute photoionization cross-section of the propargyl radical
Energy Technology Data Exchange (ETDEWEB)
Savee, John D.; Welz, Oliver; Taatjes, Craig A.; Osborn, David L. [Sandia National Laboratories, Combustion Research Facility, Livermore, California 94551 (United States); Soorkia, Satchin [Institut des Sciences Moleculaires d' Orsay, Universite Paris-Sud 11, Orsay (France); Selby, Talitha M. [Department of Chemistry, University of Wisconsin, Washington County Campus, West Bend, Wisconsin 53095 (United States)
2012-04-07
Using synchrotron-generated vacuum-ultraviolet radiation and multiplexed time-resolved photoionization mass spectrometry we have measured the absolute photoionization cross-section for the propargyl (C{sub 3}H{sub 3}) radical, {sigma}{sub propargyl}{sup ion}(E), relative to the known absolute cross-section of the methyl (CH{sub 3}) radical. We generated a stoichiometric 1:1 ratio of C{sub 3}H{sub 3} : CH{sub 3} from 193 nm photolysis of two different C{sub 4}H{sub 6} isomers (1-butyne and 1,3-butadiene). Photolysis of 1-butyne yielded values of {sigma}{sub propargyl}{sup ion}(10.213 eV)=(26.1{+-}4.2) Mb and {sigma}{sub propargyl}{sup ion}(10.413 eV)=(23.4{+-}3.2) Mb, whereas photolysis of 1,3-butadiene yielded values of {sigma}{sub propargyl}{sup ion}(10.213 eV)=(23.6{+-}3.6) Mb and {sigma}{sub propargyl}{sup ion}(10.413 eV)=(25.1{+-}3.5) Mb. These measurements place our relative photoionization cross-section spectrum for propargyl on an absolute scale between 8.6 and 10.5 eV. The cross-section derived from our results is approximately a factor of three larger than previous determinations.
Commodo, Mario; Sgro, Lee Anne; Minutolo, Patrizia; D'Anna, Andrea
2013-05-16
Photoelectric charging of particles is a powerful tool for online characterization of submicrometer aerosol particles. Indeed photoionization based techniques have high sensitivity and chemical selectivity. Moreover, they yield information on electronic properties of the material and are sensitive to the state of the surface. In the present study the photoionization charging efficiency, i.e., the ratio between the generated positive ions and the corresponding neutral ones, for different classes of flame-generated carbonaceous nanoparticles was measured. The fifth harmonics of a Nd:YAG laser, 213 nm (5.82 eV), was used as an ionization source for the combustion generated nanoparticles, whereas a differential mobility analyzer (DMA) coupled to a Faraday cup electrometer was used for particle classification and detection. Carbonaceous nanoparticles in the nucleation mode, i.e., sizes ranging from 1 to 10 nm, show a photoionization charging efficiency clearly dependent on the flame conditions. In particular, we observed that the richer the flame is, i.e., the higher the equivalent ratio is, the higher the photon charging efficiency is. We hypothesized that such an increase in the photoionization propensity of the carbonaceous nanoparticles from richer flame condition is associated to the presence within the particles of larger aromatic moieties. The results clearly show that photoionization is a powerful diagnostic tool for the physical-chemical characterization of combustion aerosol, and it may lead to further insights into the soot formation mechanism.
Impact of red giant/AGB winds on active galactic nucleus jet propagation
Perucho, M.; Bosch-Ramon, V.; Barkov, M. V.
2017-10-01
Context. Dense stellar winds may mass-load the jets of active galactic nuclei, although it is unclear on what time and spatial scales the mixing takes place. Aims: Our aim is to study the first steps of the interaction between jets and stellar winds, and also the scales on which the stellar wind mixes with the jet and mass-loads it. Methods: We present a detailed 2D simulation - including thermal cooling - of a bubble formed by the wind of a star designed to study the initial stages of jet-star interaction. We also study the first interaction of the wind bubble with the jet using a 3D simulation in which the star enters the jet. Stability analysis is carried out for the shocked wind structure to evaluate the distances over which the jet-dragged wind, which forms a tail, can propagate without mixing with the jet flow. Results.The 2D simulations point to quick wind bubble expansion and fragmentation after about one bubble shock crossing time. Three-dimensional simulations and stability analysis point to local mixing in the case of strong perturbations and relatively low density ratios between the jet and the jet dragged-wind, and to a possibly more stable shocked wind structure at the phase of maximum tail mass flux. Analytical estimates also indicate that very early stages of the star jet-penetration time may be also relevant for mass-loading. The combination of these and previous results from the literature suggests highly unstable interaction structures and efficient wind-jet flow mixing on the scale of the jet interaction height. Conclusions: The winds of stars with strong mass loss can efficiently mix with jets from active galactic nuclei. In addition, the initial wind bubble shocked by the jet leads to a transient, large interaction surface. The interaction between jets and stars can produce strong inhomogeneities within the jet. As mixing is expected to be effective on large scales, even individual asymptotic giant branch stars can significantly contribute to
Kallman, T.
2010-01-01
Warm absorber spectra are characterized by the many lines from partially ionized intermediate-Z elements, and iron, detected with the grating instruments on Chandra and XMM-Newton. If these ions are formed in a gas which is in photoionization equilibrium, they correspond to a broad range of ionization parameters, although there is evidence for certain preferred values. A test for any dynamical model for these outflows is to reproduce these properties, at some level of detail. In this paper we present a statistical analysis of the ionization distribution which can be applied both the observed spectra and to theoretical models. As an example, we apply it to our dynamical models for warm absorber outflows, based on evaporation from the molecular torus.
Kozlowski, Pawel M.; Mancini, Roberto C.; Koepke, Mark E.
2018-01-01
Many astrophysical environments such as X-ray binaries, active galactic nuclei, and accretion disks of compact objects have photoionized plasmas. The strong photoionizing environment found near these bright X-ray sources can be produced in a scaled laboratory experiment, and direct measurements can form a testbed for spectroscopic models and photoionization codes used in analysis of these astrophysical objects. Such scaled experiments are currently being conducted using Ne filled gas cells on...
Resonances in photoionization. Cross section for vibrationally excited H2
International Nuclear Information System (INIS)
Mezei, J.Zs.; Jungen, Ch.
2011-01-01
Complete text of publication follows. Diatomic molecular Hydrogen is the most abundant molecule in interstellar molecular clouds. The modeling of these environments relies on accurate cross sections for the various relevant processes. Among them, the photoionization plays a major role in the kinetics and in the energy exchanges involving H 2 . The recent discovery of vibrationally excited molecular hydrogen in extragalactic environments revealed the need for accurate evaluation of the corresponding photoionization cross sections. In the present work we report theoretical photoionization cross sections for excitation from excited vibrational levels of the ground state, dealing with the Q(N = 1) (ΔN = 0, where N is the total angular momentum of the molecule) transitions which account for roughly one third of the total photoabsorption cross section. We will focus on the v' = 1 excited level of the ground electronic state. Our calculations are based on Multichannel Quantum Defect Theory (MQDT), which allows us to take into account of the full manifold of Rydberg states and their interactions with the electronic continuum. We have carried out two types of MQDT calculations. First, we omitted all open channels and calculated energy levels, wave functions and spontaneous emission Einstein coefficients, making use of the theoretical method presented in [2]. In a second set of calculations we included the open ionization channels in the computations getting the continuum phase shifts, channel mixing coefficients and channel dipole moments and finally the photoabsorption/ photoionization cross section. The cross section is dominated by the presence of resonance structures corresponding to excitation of various vibrational levels of bound electronic states which lie above the ionization threshold. In order to assess the importance of the resonances we have calculated for each vibrational interval (the energy interval between two consecutive ionization thresholds) the
A VUV photoionization organic aerosol mass spectrometric study with synchrotron radiation
Energy Technology Data Exchange (ETDEWEB)
Fang Wenzheng; Lei Gong; Shan Xiaobin; Liu Fuyi [School of Nuclear Science and Technology, National Synchrotron Radiation Laboratory, University of Science and Technology of China, Anhui, Hefei 230029 (China); Wang Zhenya [Laboratory of Environmental Spectroscopy, Anhui Institute of Optics and Fine Mechanics, Chinese Academy of Sciences, Hefei 230031 (China); Sheng Liusi, E-mail: lssheng@ustc.edu.cn [School of Nuclear Science and Technology, National Synchrotron Radiation Laboratory, University of Science and Technology of China, Anhui, Hefei 230029 (China)
2011-04-15
Research highlights: {yields} A photoionization aerosol time-of-flight mass spectrometer (ATOFMS) has been developed for on-line analysis of organic compounds in aerosol particles using tunable vacuum ultraviolet (VUV) synchrotron radiation. {yields} The degree of fragmentation of molecule can be controlled either by the heater temperature or by the photon energy. {yields} The direct determination of the IEs of benzopheneone (9.07 eV), salicylic acid (8.72 eV), and urea (9.85 eV) are measured from the photoionization efficiency spectra. {yields} The species can be identified by their molecular and fragment ions weights as well as by the comparisions between their theoretical and experimental ionization energies. - Abstract: A photoionization aerosol time-of-flight mass spectrometer (ATOFMS) has been developed for on-line analysis of organic compounds in aerosol particles using tunable vacuum ultraviolet (VUV) synchrotron radiation. Aerosol particles can be sampled directly from atmospheric pressure and are focused through an aerodynamic lens assembly into the mass spectrometer. The particles are vaporized when they impact on a heater, and then the nascent vapor is softly photoionized by synchrotron radiation. The degree of fragmentation of molecule can be controlled either by the heater temperature or by the photon energy. Thus, fragment-free tunable VUV mass spectra are obtained by tuning the photon energy close to the ionization energies (IEs) of the sample molecules. The direct determination of the IEs of benzophenone (9.07 eV), salicylic acid (8.72 eV), and urea (9.85 eV) are measured from the photoionization efficiency spectra with uncertainties of {+-}50 meV. Ab initio calculations have been employed to predict the theoretical ionization energy.
International Nuclear Information System (INIS)
Yonekura, Nobuaki; Nakajima, Takashi; Matsuo, Yukari; Kobayashi, Tohru; Fukuyama, Yoshimitsu
2004-01-01
We report the detailed experimental study on the production of electron-spin-polarized Sr + ions through one-photon resonant two-photon ionization via laser-excited 5s5p 3 P 1 (M J =+1) of Sr atoms produced by laser-ablation. We have experimentally confirmed that the use of laser-ablation for the production of Sr atoms prior to photoionization does not affect the electron-spin polarization. We have found that the degree of electron-spin polarization is 64±9%, which is in good agreement with our recent theoretical prediction. As we discuss in detail, we infer, from a simple analysis, that photoelectrons, being the counterpart of electron-spin-polarized Sr + ions, have approximately the same degree of electron-spin polarization. Our experimental results demonstrate that the combined use of laser-ablation technique and pulsed lasers for photoionization would be a compact and effective way to realize a pulsed source for spin-polarized ions and electrons for the studies of various spin-dependent dynamics in chemical physics
Stellar Physics 2: Stellar Evolution and Stability
Bisnovatyi-Kogan, Gennady S
2011-01-01
"Stellar Physics" is a an outstanding book in the growing body of literature on star formation and evolution. Not only does the author, a leading expert in the field, very thoroughly present the current state of knowledge on stellar physics, but he handles with equal care the many problems that this field of research still faces. A bibliography with well over 1000 entries makes this book an unparalleled reference source. "Stellar Evolution and Stability" is the second of two volumes and can be read, as can the first volume "Fundamental Concepts and Stellar Equilibrium," as a largely independent work. It traces in great detail the evolution of protostars towards the main sequence and beyond this to the last stage of stellar evolution, with the corresponding vast range from white dwarfs to supernovae explosions, gamma-ray bursts and black hole formation. The book concludes with special chapters on the dynamical, thermal and pulsing stability of stars. This second edition is carefully updated in the areas of pre...
Photoion Auger-electron coincidence measurements near threshold
International Nuclear Information System (INIS)
Levin, J.C.; Biedermann, C.; Keller, N.; Liljeby, L.; Short, R.T.; Sellin, I.A.; Lindle, D.W.
1990-01-01
The vacancy cascade which fills an atomic inner-shell hole is a complex process which can proceed by a variety of paths, often resulting in a broad distribution of photoion charge states. We have measured simplified argon photoion charge distributions by requiring a coincidence with a K-LL or K-LM Auger electron, following K excitation with synchrotron radiation, as a function of photon energy, and report here in detail the argon charge distributions coincident with K-L 1 L 23 Auger electrons. The distributions exhibit a much more pronounced photon-energy dependence than do the more complicated non-coincident spectra. Resonant excitation of the K electron to np levels, shakeoff of these np electrons by subsequent decay processes, double-Auger decay, and recapture of the K photoelectron through postcollision interaction occur with significant probability. 17 refs
Double photoionization of lithium at medium energies
International Nuclear Information System (INIS)
Wehlitz, R.; Bluett, J.B.; Martinez, M.M.; Lukic, D.; Whitfield, S.B.
2004-01-01
Full text: The double-to-single photoionization ratio of atomic lithium has been measured for photon energies ranging from 120 eV to 910 eV . Through the extensive use of various filters we were able to significantly extend the previous range of measurements. We d that our data are in agreement with the predicted high-energy limit of 3.4%. By applying simple model curves to our data, we attempt to disentangle the different processes leading to a doubly charged Li ion. Our model corroborates the notion that sequential processes contribute substantially to the double-photoionization cross-section ratio as predicted by theory. This work was supported by NSF under Grant No. PHY-9987638. The SRC is supported by NSF Grant No. DMR-0084402. M.M.M. acknowledges financial support through the NSF REU program
DISSOCIATIVE PHOTOIONIZATION OF POLYCYCLIC AROMATIC HYDROCARBON MOLECULES CARRYING AN ETHYNYL GROUP
Energy Technology Data Exchange (ETDEWEB)
Rouillé, G.; Krasnokutski, S. A.; Fulvio, D.; Jäger, C. [Laboratory Astrophysics Group of the Max Planck Institute for Astronomy at the Friedrich Schiller University Jena, Institute of Solid State Physics, Helmholtzweg 3, D-07743 Jena (Germany); Henning, Th. [Max Planck Institute for Astronomy, Königstuhl 17, D-69117 Heidelberg (Germany); Garcia, G. A.; Tang, X.-F.; Nahon, L., E-mail: cornelia.jaeger@uni-jena.de [Synchrotron SOLEIL, L’Orme des Merisiers, Saint-Aubin BP 48, F-91192 Gif-sur-Yvette Cedex (France)
2015-09-10
The life cycle of the population of interstellar polycyclic aromatic hydrocarbon (PAH) molecules depends partly on the photostability of the individual species. We have studied the dissociative photoionization of two ethynyl-substituted PAH species, namely, 9-ethynylphenanthrene and 1-ethynylpyrene. Their adiabatic ionization energy and the appearance energy of fragment ions have been measured with the photoelectron photoion coincidence spectroscopy technique. The adiabatic ionization energy has been found at 7.84 ± 0.02 eV for 9-ethynylphenanthrene and at 7.41 ± 0.02 eV for 1-ethynylpyrene. These values are similar to those determined for the corresponding non-substituted PAH molecules phenanthrene and pyrene. The appearance energy of the fragment ion indicative of the loss of a H atom following photoionization is also similar for either ethynyl-substituted PAH molecule and its non-substituted counterpart. The measurements are used to estimate the critical energy for the loss of a H atom by the PAH cations and the stability of ethynyl-substituted PAH molecules upon photoionization. We conclude that these PAH derivatives are as photostable as the non-substituted species in H i regions. If present in the interstellar medium, they may play an important role in the growth of interstellar PAH molecules.
GALAXY INTERACTIONS IN COMPACT GROUPS. I. THE GALACTIC WINDS OF HCG16
Energy Technology Data Exchange (ETDEWEB)
Vogt, Frederic P. A.; Dopita, Michael A.; Kewley, Lisa J., E-mail: fvogt@mso.anu.edu.au [Mount Stromlo Observatory, Research School of Astronomy and Astrophysics, Australian National University, Cotter Road, Weston Creek, ACT 2611 (Australia)
2013-05-10
Using the WiFeS integral field spectrograph, we have undertaken a series of observations of star-forming galaxies in compact groups. In this first paper dedicated to the project, we present the analysis of the spiral galaxy NGC 838, a member of the Hickson Compact Group 16, and of its galactic wind. Our observations reveal that the wind forms an asymmetric, bipolar, rotating structure, powered by a nuclear starburst. Emission line ratio diagnostics indicate that photoionization is the dominant excitation mechanism at the base of the wind. Mixing from slow shocks (up to 20%) increases further out along the outflow axis. The asymmetry of the wind is most likely caused by one of the two lobes of the wind bubble bursting out of its H I envelope, as indicated by line ratios and radial velocity maps. The characteristics of this galactic wind suggest that it is caught early (a few Myr) in the wind evolution sequence. The wind is also quite different from the galactic wind in the partner galaxy NGC 839 which contains a symmetric, shock-excited wind. Assuming that both galaxies have similar interaction histories, the two different winds must be a consequence of the intrinsic properties of NGC 838 and NGC 839 and their starbursts.
Swank, J.
2011-01-01
Most of the stellar end-state black holes, pulsars, and white dwarfs that are X-ray sources should have polarized X-ray fluxes. The degree will depend on the relative contributions of the unresolved structures. Fluxes from accretion disks and accretion disk corona may be polarized by scattering. Beams and jets may have contributions of polarized emission in strong magnetic fields. The Gravity and Extreme Magnetism Small Explorer (GEMS) will study the effects on polarization of strong gravity of black holes and strong magnetism of neutron stars. Some part of the flux from compact stars accreting from companion stars has been reflected from the companion, its wind, or accretion streams. Polarization of this component is a potential tool for studying the structure of the gas in these binary systems. Polarization due to scattering can also be present in X-ray emission from white dwarf binaries and binary normal stars such as RS CVn stars and colliding wind sources like Eta Car. Normal late type stars may have polarized flux from coronal flares. But X-ray polarization sensitivity is not at the level needed for single early type stars.
A large stellarator based on modular coils
International Nuclear Information System (INIS)
Hamberger, S.M.; Sharp, L.E.; Petersen, L.F.
1979-06-01
Although stellarators offer some considerable advantages over tokamaks, difficulties arise in designing large devices due, for instance, to poor plasma access as well as to constructional electromechanical and maintenance problems associated with continous helical windings. This paper describes a design for a fairly large device (major radius 2.1m), based on a set of discrete coil modules arranged in a toroidal configuration to provide the required closed magnetic surfaces, having gaps for unobstructed access to the plasma for diagnostics, etc, and allowing for easy removal for maintenance
Photoionization of disk galaxies: An explanation of the sharp edges in the H I distribution
Dove, James B.; Shull, J. Michael
1994-01-01
We have reproduced the observed radial truncation of the H I distribution in isolated spiral galaxies with a model in which extragalactic radiation photoionizes the gaseous disk. For a galactic mass distribution model that reproduces the observed rotation curves, including dark matter in the disk and halo, the vertical structure of the gas is determined self-consistently. The ionization structure and column densities of H and He ions are computed by solving the radiation transfer equation for both continuum and lines. Our model is similar to that of Maloney, and the H I structure differs by less than 10%. The radial structure of the column density of H I is found to be more sensitive to the extragalactic radiation field than to the distribution of mass. For this reason, considerable progress can be made in determining the extragalactic flux of ionizing photons, phi(sub ex), with more 21 cm observations of isolated galaxies. However, owing to the uncertainty of the radial distribution of total hydrogen at large radii, inferring the extragalactic flux by comparing the observed edges to photoionization models is somewhat subjective. We find 1 x 10(exp 4)/sq cm/s is less than or approximately phi(sub ex) is less than or approximately 5 x 10(exp 4)/sq cm/s, corresponding to 2.1 is less than or approximately iota(sub 0) is less than or approximately 10.5 x 10(exp -23) ergs/sq cm/s/Hz/sr for a 1/nu spectrum. Although somewhat higher, our inferred range of iota(sub 0) is consistent with the large range of values obtained by Kulkarni & Fall from the 'proximity effect' toward Quasi-Stellar Objects (QSOs) at approximately 0.5.
International Nuclear Information System (INIS)
Burileanu, L.M.
2014-01-01
Using a perturbative method we have investigated the behavior of the binding energy and photoionization cross-section of a donor impurity in spherical GaAs–GaAlAs quantum dots under the influence of electric and intense high-frequency laser fields. The dependencies of the binding energy and photoionization cross-section on electric and laser field strength, dot radius and impurity position were investigated. Our results show that the amplitude of photoionization cross-section grows with the dot radius increase and the peak of the cross-section blue shifts with the laser intensity increment. We have found that the binding energy is not a monotonically function of laser intensity: it decreases or increases depending on electric field regime. The studied effects are even more pronounced as the quantum dot radius is smaller. -- Highlights: • A photoionization cross-section study in quantum dots under laser and electric fields. • The photoionization cross-section peaks are red shifted by the electric field. • The photoionization cross-section peaks are blue shifted by the laser field. • The combined effects of applied fields strongly affect the binding energy
Double K-vacancy production by x-ray photoionization
International Nuclear Information System (INIS)
Southworth, S. H.; Dunford, R. W.; Kanter, E. P.; Krassig, B.; Young, L.; Armen, G. B.; Levin, J. C.; Chen, M. H.; Ederer, D. L.
2002-01-01
We have studied double K-shell photoionization of Ne and Mo (Z = 10 and 42) at the Advanced Photon Source. Double K-vacancy production in Ne was observed by recording the KK-KLL Auger hypersatellite spectrum. Comparison is made with calculations using the multiconfiguration Dirac-Fock method. For Mo, double K-vacancy production was observed by recording the Kα, β fluorescence hypersatellite and satellite x rays in coincidence. From the intensities of the Auger or x-ray hypersatellites relative to diagram lines, the probabilities for double K-vacancy production relative to single K-vacancies were determined. These results, along with reported measurements on other atoms, are compared with Z-scaling calculations of the high-energy limits of the double-to-single K-shell photoionization ratio
Effect of mass loss by stellar wind on the chemical enrichment of the galaxy
Energy Technology Data Exchange (ETDEWEB)
Chiosi, C [Padua Univ. (Italy). Istituto di Astronomia
1979-01-01
The rate of production of heavy elements is rediscussed using the models of Arnett (1978) for late stage nucleosynthesis in massive stars, the M(M,) relationship of Chiosi et al. (1978b) for losing mass models in the core H and He-Burning phases, and the stellar birth rate of Miller and Scalo (1978). Contrary to that found by Wheeler et al (1978), we do not encounter the difficulty of heavy element overproduction. The explosive nucleosynthesis from massive stars is still compatible with the observed abundance distribution of the solar system, and a stellar birth rate decreasing over the history of the galactic disk.
Energy Technology Data Exchange (ETDEWEB)
Bizau, J.M., E-mail: jean-marc.bizau@u-psud.fr [Institut des Sciences Moléculaires d’Orsay (ISMO), CNRS, Univ. Paris Paris-Sud, Université Paris-Saclay, F-91405 Orsay (France); Synchrotron SOLEIL, L’Orme des Merisiers, Saint-Aubin, BP 48, F-91192 Gif-sur-Yvette Cedex (France); Cubaynes, D. [Institut des Sciences Moléculaires d’Orsay (ISMO), CNRS, Univ. Paris Paris-Sud, Université Paris-Saclay, F-91405 Orsay (France); Synchrotron SOLEIL, L’Orme des Merisiers, Saint-Aubin, BP 48, F-91192 Gif-sur-Yvette Cedex (France); Guilbaud, S.; El Eassan, N.; Al Shorman, M.M.; Bouisset, E.; Guigand, J.; Moustier, O.; Marié, A.; Nadal, E. [Institut des Sciences Moléculaires d’Orsay (ISMO), CNRS, Univ. Paris Paris-Sud, Université Paris-Saclay, F-91405 Orsay (France); Robert, E.; Nicolas, C. [Synchrotron SOLEIL, L’Orme des Merisiers, Saint-Aubin, BP 48, F-91192 Gif-sur-Yvette Cedex (France); Miron, C. [Synchrotron SOLEIL, L’Orme des Merisiers, Saint-Aubin, BP 48, F-91192 Gif-sur-Yvette Cedex (France); Extreme Light Infrastructure—Nuclear Physics, “Horia Hulubei” National Institute for Physics and Nuclear Engineering, 30 Reactorului Street, RO-077125 Măgurele, Jud. Ilfov (Romania)
2016-07-15
Highlights: • Description of a merged-beam setup at SOLEIL synchrotron radiation facility. • Unique setup of this kind allowing photoelectron spectroscopy on ionic species. • Use of electron-ion coincidence to reduce the background. • Examples on the photoionization of Xe{sup 5+} multiply-charged ion. - Abstract: We describe the merged-beam setup permanently installed on a dedicated optical branch of the PLEIADES beamline at SOLEIL, the French synchrotron radiation facility in St-Aubin, delivering photons in the 10–1000 eV photon energy range. The setup is designed both for photoion and photoelectron spectroscopy experiments on atomic and molecular ions. Ion spectrometry is dedicated to the determination of absolute single and multiple photoionization cross sections. Electron spectroscopy brings additional information on the non-radiative decay of inner-vacancies produced in the photoionization processes and allows for the determination of partial cross sections. Efficient reduction of the background in the electron spectra is achieved by the use of the electron-ion coincidence technique. Examples of photoion and photoelectron spectra are given for the Xe{sup 5+} ion.
Low frequency RF heating of plasmas in a toroidal stellarator
International Nuclear Information System (INIS)
Golovato, S.N.
1977-01-01
Studies of transit-time magnetic pumping and Alfven wave heating have been done in the Proto-Cleo stellarator. Both plasma heating and plasma confinement have been investigated. A traveling wave was launched around the Proto-Cleo l = 2, 6 field period stellarator to attempt transit-time magnetic pumping of a pulsed electron beam moving along the magnetic field lines. An apparent loss of the beam was seen when the transit-time magnetic pumping was applied. A random walk diffusion of the beam electrons with a step size determined by the radial EXB drift due to the poloidal electric field agrees well with the experimental results. Alfven wave heating was applied to plasmas in the Proto-Cleo l = 3, 7 field period stellarator. Global excitation of Alfven waves was accomplished by exciting an electrostatically shielded helical winding corresponding to a q = 3 rational field line with a pulsed, high-power RF source. Theoretical analysis of this helical wave launcher predicted effective energy absorption in the Proto-Cleo gun-produced plasma
Feedback by AGN Jets and Wide-angle Winds on a Galactic Scale
Energy Technology Data Exchange (ETDEWEB)
Dugan, Zachary; Silk, Joseph [The Johns Hopkins University Department of Physics and Astronomy, Bloomberg Center for Physics and Astronomy, Room 366, 3400 N. Charles Street, Baltimore, MD 21218 (United States); Gaibler, Volker [Universität Heidelberg, Zentrum für Astronomie, Institut für Theoretische Astrophysik, Albert-Ueberle-Str. 2, D-69120 Heidelberg (Germany)
2017-07-20
To investigate the differences in mechanical feedback from radio-loud and radio-quiet active galactic nuclei on the host galaxy, we perform 3D AMR hydrodynamic simulations of wide-angle, radio-quiet winds with different inclinations on a single, massive, gas-rich disk galaxy at a redshift of 2–3. We compare our results to hydrodynamic simulations of the same galaxy but with a jet. The jet has an inclination of 0° (perpendicular to the galactic plane), and the winds have inclinations of 0°, 45°, and 90°. We analyze the impact on the host’s gas, star formation, and circumgalactic medium. We find that jet feedback is energy-driven and wind feedback is momentum-driven. In all the simulations, the jet or wind creates a cavity mostly devoid of dense gas in the nuclear region where star formation is then quenched, but we find strong positive feedback in all the simulations at radii greater than 3 kpc. All four simulations have similar SFRs and stellar velocities with large radial and vertical components. However, the wind at an inclination of 90° creates the highest density regions through ram pressure and generates the highest rates of star formation due to its ongoing strong interaction with the dense gas of the galactic plane. With increased wind inclination, we find greater asymmetry in gas distribution and resulting star formation. Our model generates an expanding ring of triggered star formation with typical velocities of the order of 1/3 of the circular velocity, superimposed on the older stellar population. This should result in a potentially detectable blue asymmetry in stellar absorption features at kiloparsec scales.
A new class of galactic discrete gamma ray sources: Chaotic winds of massive stars
Chen, Wan; White, Richard L.
1992-01-01
We propose a new class of galactic discrete gamma-ray sources, the chaotic, high mass-loss-rate winds from luminous early-type stars. Early-type stellar winds are highly unstable due to intrinsic line-driven instabilities, and so are permeated by numerous strong shocks. These shocks can accelerate a small fraction of thermal electrons and ions to relativistic energies via the first-order Fermi mechanism. A power-law-like photon spectrum extending from keV to above 10 MeV energies is produced by inverse Compton scattering of the extremely abundant stellar UV photons by the relativistic electrons. In addition, a typical pi(sup 0)-decay gamma-ray spectrum is generated by proton-ion interactions in the densest part of the winds.
Atomic Physics of Shocked Plasma in Winds of Massive Stars
Leutenegger, Maurice A.; Cohen, David H.; Owocki, Stanley P.
2012-01-01
High resolution diffraction grating spectra of X-ray emission from massive stars obtained with Chandra and XMM-Newton have revolutionized our understanding of their powerful, radiation-driven winds. Emission line shapes and line ratios provide diagnostics on a number of key wind parameters. Modeling of resolved emission line velocity profiles allows us to derive independent constraints on stellar mass-loss rates, leading to downward revisions of a factor of a few from previous measurements. Line ratios in He-like ions strongly constrain the spatial distribution of Xray emitting plasma, confirming the expectations of radiation hydrodynamic simulations that X-ray emission begins moderately close to the stellar surface and extends throughout the wind. Some outstanding questions remain, including the possibility of large optical depths in resonance lines, which is hinted at by differences in line shapes of resonance and intercombination lines from the same ion. Resonance scattering leads to nontrivial radiative transfer effects, and modeling it allows us to place constraints on shock size, density, and velocity structure
Photoionization cross-section of shallow donors impurities at all magnetic fields
International Nuclear Information System (INIS)
Zorkani, I.; Filali, L.
1998-09-01
The dependence of the photoionization cross-section for shallow donors on photon energy is calculated. The effects of strong and weak magnetic fields are considered by means of a variational wave function which is a linear combination of the cylindrical wave function and the oscillator one. Simple analytical expressions, valid for all magnetic fields, are obtained. It has been found that the photoionization cross-section is affected by the magnetic field. We give some results of Germanium. (author)
Multiple photoionization following 3d5/2-shell threshold ionization of
International Nuclear Information System (INIS)
Matsui, T; Yoshii, H; Tsukamoto, K; Kawakita, S; Murakami, E; Adachi, J; Yagishita, A; Morioka, Y; Hayaishi, T
2004-01-01
Multiple photoionization of Xe near the 3d 5/2 -shell threshold photoionization region is studied by threshold electron-ion coincidence spectroscopy. The coincidence spectra of Xe 3+ to Xe 7+ ions exhibit characteristic profiles associated with multi-step post-collision interactions in Auger cascades following 3d 5/2 -shell threshold photoionization. The Auger cascade decay channels leading to the formation of multiply charged ions are deduced from the energies of the profile peaks, which increase gradually with increasing charge state. The formation of Xe 3+ to Xe 5+ ions is found to arise from cascades of normal Auger decays, whereas the formation of Xe 6+ and Xe 7+ ions involves double Auger decays. The branching ratio of double to normal Auger decays is estimated to be 0.25 (±0.1) for the decays following the creation of 3d 5/2 -hole states in Xe
New photoionization models of intergalactic clouds
Donahue, Megan; Shull, J. M.
1991-01-01
New photoionization models of optically thin low-density intergalactic gas at constant pressure, photoionized by QSOs, are presented. All ion stages of H, He, C, N, O, Si, and Fe, plus H2 are modeled, and the column density ratios of clouds at specified values of the ionization parameter of n sub gamma/n sub H and cloud metallicity are predicted. If Ly-alpha clouds are much cooler than the previously assumed value, 30,000 K, the ionization parameter must be very low, even with the cooling contribution of a trace component of molecules. If the clouds cool below 6000 K, their final equilibrium must be below 3000 K, owing to the lack of a stable phase between 6000 and 3000 K. If it is assumed that the clouds are being irradiated by an EUV power-law continuum typical of WSOs, with J0 = 10 exp -21 ergs/s sq cm Hz, typical cloud thicknesses along the line of sight that are much smaller than would be expected from shocks, thermal instabilities, or gravitational collapse are derived.
Recent advances in stellarator optimization
Gates, D. A.; Boozer, A. H.; Brown, T.; Breslau, J.; Curreli, D.; Landreman, M.; Lazerson, S. A.; Lore, J.; Mynick, H.; Neilson, G. H.; Pomphrey, N.; Xanthopoulos, P.; Zolfaghari, A.
2017-12-01
Computational optimization has revolutionized the field of stellarator design. To date, optimizations have focused primarily on optimization of neoclassical confinement and ideal MHD stability, although limited optimization of other parameters has also been performed. The purpose of this paper is to outline a select set of new concepts for stellarator optimization that, when taken as a group, present a significant step forward in the stellarator concept. One of the criticisms that has been leveled at existing methods of design is the complexity of the resultant field coils. Recently, a new coil optimization code—COILOPT++, which uses a spline instead of a Fourier representation of the coils,—was written and included in the STELLOPT suite of codes. The advantage of this method is that it allows the addition of real space constraints on the locations of the coils. The code has been tested by generating coil designs for optimized quasi-axisymmetric stellarator plasma configurations of different aspect ratios. As an initial exercise, a constraint that the windings be vertical was placed on large major radius half of the non-planar coils. Further constraints were also imposed that guaranteed that sector blanket modules could be removed from between the coils, enabling a sector maintenance scheme. Results of this exercise will be presented. New ideas on methods for the optimization of turbulent transport have garnered much attention since these methods have led to design concepts that are calculated to have reduced turbulent heat loss. We have explored possibilities for generating an experimental database to test whether the reduction in transport that is predicted is consistent with experimental observations. To this end, a series of equilibria that can be made in the now latent QUASAR experiment have been identified that will test the predicted transport scalings. Fast particle confinement studies aimed at developing a generalized optimization algorithm are also
International Nuclear Information System (INIS)
Montes, Gabriela; Ramirez-Ruiz, Enrico; De Colle, Fabio; Strickler, Rachel
2013-01-01
The problem of explaining the X-ray emission properties of the massive, close binary WR 20a is discussed. Located near the cluster core of Westerlund 2, WR 20a is composed of two nearly identical Wolf-Rayet stars of 82 and 83 solar masses orbiting with a period of only 3.7 days. Although Chandra observations were taken during the secondary optical eclipse, the X-ray light curve shows no signs of a flux decrement. In fact, WR 20a appears slightly more X-ray luminous and softer during the optical eclipse, opposite to what has been observed in other binary systems. To aid in our interpretation of the data, we compare with the results of hydrodynamical simulations using the adaptive mesh refinement code Mezcal which includes radiative cooling and a radiative acceleration force term. It is shown that the X-ray emission can be successfully explained in models where the wind-wind collision interface in this system occurs while the outflowing material is still being accelerated. Consequently, WR 20a serves as a critical test-case for how radiatively driven stellar winds are initiated and how they interact. Our models not only procure a robust description of current Chandra data, which cover the orbital phases between 0.3 and 0.6, but also provide detailed predictions over the entire orbit
Montes, Gabriela; Ramirez-Ruiz, Enrico; De Colle, Fabio; Strickler, Rachel
2013-11-01
The problem of explaining the X-ray emission properties of the massive, close binary WR 20a is discussed. Located near the cluster core of Westerlund 2, WR 20a is composed of two nearly identical Wolf-Rayet stars of 82 and 83 solar masses orbiting with a period of only 3.7 days. Although Chandra observations were taken during the secondary optical eclipse, the X-ray light curve shows no signs of a flux decrement. In fact, WR 20a appears slightly more X-ray luminous and softer during the optical eclipse, opposite to what has been observed in other binary systems. To aid in our interpretation of the data, we compare with the results of hydrodynamical simulations using the adaptive mesh refinement code Mezcal which includes radiative cooling and a radiative acceleration force term. It is shown that the X-ray emission can be successfully explained in models where the wind-wind collision interface in this system occurs while the outflowing material is still being accelerated. Consequently, WR 20a serves as a critical test-case for how radiatively driven stellar winds are initiated and how they interact. Our models not only procure a robust description of current Chandra data, which cover the orbital phases between 0.3 and 0.6, but also provide detailed predictions over the entire orbit.
Energy Technology Data Exchange (ETDEWEB)
Montes, Gabriela; Ramirez-Ruiz, Enrico; De Colle, Fabio; Strickler, Rachel [Department of Astronomy and Astrophysics, University of California, Santa Cruz, CA 95064 (United States)
2013-11-10
The problem of explaining the X-ray emission properties of the massive, close binary WR 20a is discussed. Located near the cluster core of Westerlund 2, WR 20a is composed of two nearly identical Wolf-Rayet stars of 82 and 83 solar masses orbiting with a period of only 3.7 days. Although Chandra observations were taken during the secondary optical eclipse, the X-ray light curve shows no signs of a flux decrement. In fact, WR 20a appears slightly more X-ray luminous and softer during the optical eclipse, opposite to what has been observed in other binary systems. To aid in our interpretation of the data, we compare with the results of hydrodynamical simulations using the adaptive mesh refinement code Mezcal which includes radiative cooling and a radiative acceleration force term. It is shown that the X-ray emission can be successfully explained in models where the wind-wind collision interface in this system occurs while the outflowing material is still being accelerated. Consequently, WR 20a serves as a critical test-case for how radiatively driven stellar winds are initiated and how they interact. Our models not only procure a robust description of current Chandra data, which cover the orbital phases between 0.3 and 0.6, but also provide detailed predictions over the entire orbit.
Schwell, Martin; Bé nilan, Yves; Fray, Nicolas; Gazeau, Marie Claire; Es-sebbar, Et-touhami; Garcí a, Gustavo A.; Nahon, Laurent; Champion, Norbert; Leach, Sydney Sydney
2012-01-01
A VUV photoionization study of acetamide was carried out over the 8-24 eV photon energy range using synchrotron radiation and photoelectron/photoion coincidence (PEPICO) spectroscopy. Threshold photoelectron photoion coincidence (TPEPICO) measurements were also made. Photoion yield curves and branching ratios were measured for the parent ion and six fragment ions. The adiabatic ionization energy of acetamide was determined as I.E. (1 2A′) = (9.71 ± 0.02) eV, in agreement with an earlier reported photoionization mass spectrometry (PIMS) value. The adiabatic energy of the first excited state of the ion, 1 2A″, was determined to be ≈10.1 eV. Assignments of the fragment ions and the pathways of their formation by dissociative photoionization were made. The neutral species lost in the principal dissociative photoionization processes are CH 3, NH 2, NH 3, CO, HCCO and NH 2CO. Heats of formation are derived for all ions detected and are compared with literature values. Some astrophysical implications of these results are discussed. © 2011 Elsevier B.V. All rights reserved.
Keilbach, D.; Drews, C.; Taut, A.; Wimmer-Schweingruber, R. F.
2016-12-01
Recent studies of the inflow direction of the local insterstellar medium from PUI density distributions have shown that the extrema of the longitudinal distribution of PUI velocities (with respect to the solar wind speed) can be attributed to the radial velocity of the interstellar neutral seed population and is symmetric around the inflow direction of the local interstellar medium. This work is aimed to model pickup ion injection rates from photoionization (which is the main process of interstellar PUI production) throughout the heliosphere. To that end a seed population of interstellar neutrals is injected into a model heliosphere at 60 AU distance from the sun, whereas each particle's initial speed is given by a maxwellian distribution at a temperature of 1 eV and an inflow speed of 22 km/s. Then the density of the interstellar neutrals is integrated over the model heliosphere, while the movement of the neutrals is simulated using timestep methods. To model the focusing of the interstellar neutral trajectories from the sun's gravitational potential the model heliosphere contains a central gravitational potential.Each neutral test particle can be ionized via photoionization with a per-timestep probability antiproportional to the neutral's distance to the sun squared. By tracking the ionization rate location-dependently, PUI injection rates have been determined. Therefore using these simulations the density distributions of different species of interstellar neutrals have been calculated. In addition location-dependent injection rates of different species of PUIs have been calculated, which show an increased rate of PUI production in the focusing cone region (e.g. for He+ PUIs), but also in the crescent region (e.g. for O+ PUIs).Furthermore the longitudinal distribution of the neutrals' velocity at 1 AU is calculated from the simulation's results in order to estimate the PUI cut-off as a function of ecliptic longitude. Figure: Simulated He neutral density (left
RECONSTRUCTING THE SOLAR WIND FROM ITS EARLY HISTORY TO CURRENT EPOCH
Energy Technology Data Exchange (ETDEWEB)
Airapetian, Vladimir S.; Usmanov, Arcadi V., E-mail: vladimir.airapetian@nasa.gov, E-mail: avusmanov@gmail.com [NASA Goddard Space Flight Center, Greenbelt, MD (United States)
2016-02-01
Stellar winds from active solar-type stars can play a crucial role in removal of stellar angular momentum and erosion of planetary atmospheres. However, major wind properties except for mass-loss rates cannot be directly derived from observations. We employed a three-dimensional magnetohydrodynamic Alfvén wave driven solar wind model, ALF3D, to reconstruct the solar wind parameters including the mass-loss rate, terminal velocity, and wind temperature at 0.7, 2, and 4.65 Gyr. Our model treats the wind thermal electrons, protons, and pickup protons as separate fluids and incorporates turbulence transport, eddy viscosity, turbulent resistivity, and turbulent heating to properly describe proton and electron temperatures of the solar wind. To study the evolution of the solar wind, we specified three input model parameters, the plasma density, Alfvén wave amplitude, and the strength of the dipole magnetic field at the wind base for each of three solar wind evolution models that are consistent with observational constrains. Our model results show that the velocity of the paleo solar wind was twice as fast, ∼50 times denser and 2 times hotter at 1 AU in the Sun's early history at 0.7 Gyr. The theoretical calculations of mass-loss rate appear to be in agreement with the empirically derived values for stars of various ages. These results can provide realistic constraints for wind dynamic pressures on magnetospheres of (exo)planets around the young Sun and other active stars, which is crucial in realistic assessment of the Joule heating of their ionospheres and corresponding effects of atmospheric erosion.
RECONSTRUCTING THE SOLAR WIND FROM ITS EARLY HISTORY TO CURRENT EPOCH
International Nuclear Information System (INIS)
Airapetian, Vladimir S.; Usmanov, Arcadi V.
2016-01-01
Stellar winds from active solar-type stars can play a crucial role in removal of stellar angular momentum and erosion of planetary atmospheres. However, major wind properties except for mass-loss rates cannot be directly derived from observations. We employed a three-dimensional magnetohydrodynamic Alfvén wave driven solar wind model, ALF3D, to reconstruct the solar wind parameters including the mass-loss rate, terminal velocity, and wind temperature at 0.7, 2, and 4.65 Gyr. Our model treats the wind thermal electrons, protons, and pickup protons as separate fluids and incorporates turbulence transport, eddy viscosity, turbulent resistivity, and turbulent heating to properly describe proton and electron temperatures of the solar wind. To study the evolution of the solar wind, we specified three input model parameters, the plasma density, Alfvén wave amplitude, and the strength of the dipole magnetic field at the wind base for each of three solar wind evolution models that are consistent with observational constrains. Our model results show that the velocity of the paleo solar wind was twice as fast, ∼50 times denser and 2 times hotter at 1 AU in the Sun's early history at 0.7 Gyr. The theoretical calculations of mass-loss rate appear to be in agreement with the empirically derived values for stars of various ages. These results can provide realistic constraints for wind dynamic pressures on magnetospheres of (exo)planets around the young Sun and other active stars, which is crucial in realistic assessment of the Joule heating of their ionospheres and corresponding effects of atmospheric erosion
International Nuclear Information System (INIS)
Hakimifard, A.
2010-01-01
The effect of the donor impurity position and the form of confining potential on the binding energy and the photoionization cross-section if a semiconductor quantum well with Poschl-Teller potential is investigated. An analytical expression for the photoionization cross-section is obtained for the case when the polarization vector of light wave is directed along the direction of size quantization. It is shown that the photoionization cross-section has a threshold behavior
Magnetized Disk Winds in NGC 3783
Fukumura, Keigo; Kazanas, Demosthenes; Shrader, Chris; Behar, Ehud; Tombesi, Francesco; Contopoulos, Ioannis
2018-01-01
We analyze a 900 ks stacked Chandra/HETG spectrum of NGC 3783 in the context of magnetically driven accretion-disk wind models in an effort to provide tight constraints on the global conditions of the underlying absorbers. Motivated by the earlier measurements of its absorption measure distribution (AMD) indicating X-ray-absorbing ionic columns that decrease slowly with decreasing ionization parameter, we employ 2D magnetohydrodynamic (MHD) disk wind models to describe the global outflow. We compute its photoionization structure along with the wind kinematic properties, allowing us to further calculate in a self-consistent fashion the shapes of the major X-ray absorption lines. With the wind radial density profile determined by the AMD, the profiles of the ensemble of the observed absorption features are determined by the two global parameters of the MHD wind; i.e., disk inclination {θ }{obs} and wind density normalization n o . Considering the most significant absorption features in the ∼1.8–20 Å range, we show that the MHD wind is best described by n{(r)∼ 6.9× {10}11(r/{r}o)}-1.15 cm‑3 and {θ }{obs}=44^\\circ . We argue that winds launched by X-ray heating or radiation pressure, or even MHD winds but with steeper radial density profiles, are strongly disfavored by data. Considering the properties of Fe K-band absorption features (i.e., Fe XXV and Fe XXVI), while typically prominent in the active galactic nucleus X-ray spectra, they appear to be weak in NGC 3783. For the specific parameters of our model obtained by fitting the AMD and the rest of the absorption features, these features are found to be weak, in agreement with observations.
Double-photoionization of helium including quadrupole radiation effects
Energy Technology Data Exchange (ETDEWEB)
Colgan, James [Los Alamos National Laboratory; Ludlow, J A [AUBURN UNIV; Lee, Teck - Ghee [AUBURN UNIV; Pindzola, M S [AUBURN UNIV; Robicheaux, F [AUBURN UNIV
2009-01-01
Non-perturbative time-dependent close-coupling calculations are carried out for the double photoionization of helium including both dipole and quadrupole radiation effects. At a photon energy of 800 eV, accessible at CUlTent synchrotron light sources, the quadrupole interaction contributes around 6% to the total integral double photoionization cross section. The pure quadrupole single energy differential cross section shows a local maxima at equal energy sharing, as opposed to the minimum found in the pure dipole single energy differential cross section. The sum of the pure dipole and pure quadrupole single energy differentials is insensitive to non-dipole effects at 800 eV. However, the triple differential cross section at equal energy sharing of the two ejected electrons shows strong non-dipole effects due to the quadrupole interaction that may be experimentally observable.
Double-Exponentially Decayed Photoionization in CREI Effect: Numerical Experiment on 3D H2+
International Nuclear Information System (INIS)
Feng, Li; Ting-Ying, Wang; Gui-Zhong, Zhang; Wang-Hua, Xiang; III, W. T. Hill
2008-01-01
On the platform of the 3D H 2 + system, we perform a numerical simulation of its photoionization rate under excitation of weak to intense laser intensities with varying pulse durations and wavelengths. A novel method is proposed for calculating the photoionization rate: a double exponential decay of ionization probability is best suited for fitting this rate. Confirmation of the well-documented charge-resonance-enhanced ionization (CREI) effect at medium laser intensity and finding of ionization saturation at high light intensity corroborate the robustness of the suggested double-exponential decay process. Surveying the spatial and temporal variations of electron wavefunctions uncovers a mechanism for the double-exponentially decayed photoionization probability as onset of electron ionization along extra degree of freedom. Henceforth, the new method makes clear the origins of peak features in photoionization rate versus internuclear separation. It is believed that this multi-exponentially decayed ionization mechanism is applicable to systems with more degrees of motion
Photoionization of the 4d subshell of the La isonuclear sequence
Kalyadan, Sindhu; Varma, Hari R.; Deshmukh, P. C.; Costello, J. T.; Hayden, P.; Manson, S. T.
2015-05-01
Photoionization studies along isonuclear sequences provide the required systematic data which are useful in many practical applications and also for testing the accuracy of various theoretical models. In the present work, we report on 4d subshell photoionization studies of some of the members of La (Z = 57) isonuclear sequence (La3+, La9+ and La11+) using relativistic random phase approximation (RRPA). Photoionization cross sections, σ, angular distribution asymmetry parameters, β, and the individual dipole matrix elements for 4d3/2 and 4d5/2 subshells are presented along with the 4d branching ratios of these ions. It is found that in La3+, the branching ratios show significant departure from the statistical value 1.5 due to the presence of Cooper minimum in the 4d --> f ionization channels. This departure is minor for the case of La9+ and La11+ since the Cooper minimum in these cases occur in the discrete part of the 4d spectrum.
Photoionization of sodium atoms and electron scattering from ionized sodium
Dasgupta, A.; Bhatia, A. K.
1985-01-01
The polarized-orbital method of Temkin (1957) is applied using polarized orbitals determined from Sternheimer's equation to compute the photoionization cross sections of Na atoms from threshold to about 60 eV. The approximations involved in the analysis are explained in detail; the explicit forms of the integrals and matrix expressions are given in appendices; and the results are presented in tables and graphs. Good agreement is found with the results of Chang and Kelly (1975), and the possibility that small amounts of molecular vapor in Na-photoionization experiments are responsible for the discrepancies between calculated and measured cross sections is considered.
Intershell interaction in excited atom and ion photoionization
International Nuclear Information System (INIS)
Amusia, M.Ya.; Avdonina, N.B.
1989-01-01
It is demonstrated, that the photoionization cross section of an excited electron in Cs atom isoelectronic sequence acquire additional structure if the virtual polarization of the core by the incident photon is taken into account. (orig.)
Theoretical study on the photoionization of metanal and fluoromethane
International Nuclear Information System (INIS)
Tanaka, Helder Kenji; Silveira, Tiago Rodrigues; Nascimento, Edmar Moraes do
2011-01-01
Full text. The photoionization study of biological interest molecules has increased last few years due to the basic interest in the fundamental nature of electronic structures and scattering molecular processes. It was considered to this study hypothesis in that simple molecules would give birth to more complex molecules through photochemical reactions induced by interstellar radiation. This paper shows a theoretical study over photoionization of the valence shells of some biological interest molecules. Cross sections and parameters of asymmetry are set due to ab initio, using the continued fractions method to determine the scattering matrix and wave functions of the continuum. Results will be presented to the valence shell photoionization of formaldehyde (CH 2 O) and fluoromethane (CH 3 F). This work is part of a larger project to study of biological interest molecules, motivated by the hypothesis that based on these simple molecules, physicochemical processes may have given origin to more complex molecules responsible for the production of terrestrial life. The formamide, for example, has been subject of interest between researchers as a possible material from which can be created RNA bases. In this case has been studied the production of guanine from the formamide heated while irradiated by ultraviolet radiation
Effective temperature of an ultracold electron source based on near-threshold photoionization.
Engelen, W J; Smakman, E P; Bakker, D J; Luiten, O J; Vredenbregt, E J D
2014-01-01
We present a detailed description of measurements of the effective temperature of a pulsed electron source, based on near-threshold photoionization of laser-cooled atoms. The temperature is determined by electron beam waist scans, source size measurements with ion beams, and analysis with an accurate beam line model. Experimental data is presented for the source temperature as a function of the wavelength of the photoionization laser, for both nanosecond and femtosecond ionization pulses. For the nanosecond laser, temperatures as low as 14 ± 3 K were found; for femtosecond photoionization, 30 ± 5 K is possible. With a typical source size of 25 μm, this results in electron bunches with a relative transverse coherence length in the 10⁻⁴ range and an emittance of a few nm rad. © 2013 Elsevier B.V. All rights reserved.
Radiation-driven winds in x-ray binaries
International Nuclear Information System (INIS)
Friend, D.B.; Castor, J.I.
1982-01-01
We discuss the properties of a radiation-driven stellar wind in an X-ray binary system. The Castor, Abbott, Klein line-driven wind model is used, but the effects of the compact companion (gravity and continuum radiation pressure) and the centrifugal force due to orbital motion are included. These forces destroy the spherical symmetry of the wind and can make the mass loss and accretion strong functions of the size of the primary relative to its critical potential lobe. We in most systems the wind alone could power the X-ray emission. It also appears that, in the evolution of these systems, there would be a continuous transition from wind accretion to critical potential lobe overflow. The model is also used to make a prediction about the nature of a suspected binary system which is not known to be an X-ray emitter
Radiatively-driven winds: model improvements, ionization balance and the infared spectrum
International Nuclear Information System (INIS)
Castor, J.I.
1979-01-01
Recent improvements to theoretical stellar wind models and the results of empirical modelling of the ionization balance and the infrared continuum are discussed. The model of a wind driven by radiation pressure in spectral lines is improved by accounting for overlap of the driving lines, dependence of ionization balance on density, and stellar rotation. These effects produce a softer velocity law than that given by Castor, Abbott and Klein (1975). The ionization balance in zeta Puppis is shown to agree with that estimated for an optically thick wind at a gas temperature of 60,000 K. The ionization model is not unique. The infrared continuum of zeta Pup measured by Barlow and Cohen is fitted to a cool model with a linear rise of velocity with radius; this fit is also not unique. It is concluded that one should try to find a model that fits several kinds of evidence simultaneously. (Auth.)
Absolute photoionization cross sections of furanic fuels: 2-ethylfuran, 2-acetylfuran and furfural.
Smith, Audrey R; Meloni, Giovanni
2015-11-01
Absolute photoionization cross sections of the molecules 2-ethylfuran, 2-acetylfuran and furfural, including partial ionization cross sections for the dissociative ionized fragments, are measured for the first time. These measurements are important because they allow fuel quantification via photoionization mass spectrometry and the development of quantitative kinetic modeling for the complex combustion of potential fuels. The experiments are carried out using synchrotron photoionization mass spectrometry with an orthogonal time-of-flight spectrometer used for mass analysis at the Advanced Light Source of Lawrence Berkeley National Laboratory. The CBS-QB3 calculations of adiabatic ionization energies and appearance energies agree well with the experimental results. Several bond dissociation energies are also derived and presented. Copyright © 2015 John Wiley & Sons, Ltd.
Clumpy wind accretion in Supergiant X-ray Binaries
El Mellah, I.; Sundqvist, J. O.; Keppens, R.
2017-12-01
Supergiant X-ray binaries (\\sgx) contain a neutron star (NS) orbiting a Supergiant O/B star. The fraction of the dense and fast line-driven wind from the stellar companion which is accreted by the NS is responsible for most of the X-ray emission from those system. Classic \\sgx display photometric variability of their hard X-ray emission, typically from a few 10^{35} to a few 10^{37}erg\\cdots^{-1}. Inhomogeneities (\\aka clumps) in the wind from the star are expected to play a role in this time variability. We run 3D hydrodynamical (HD) finite volume simulations to follow the accretion of the inhomogeneous stellar wind by the NS over almost 3 orders of magnitude. To model the unperturbed wind far upstream the NS, we use recent simulations which managed to resolve its micro-structure. We observe the formation of a Bondi-Hoyle-Lyttleton (BHL) like bow shock around the accretor and follow the clumps as they cross it, down to the NS magnetosphere. Compared to previous estimations discarding the HD effects, we measure lower time variability due to both the damping effect of the shock and the necessity to evacuate angular momentum to enable accretion. We also compute the associated time-variable column density and compare it to recent observations in Vela X-1.
Calculation of the photoionization cross section of the 4d10 subshell of the La atom
International Nuclear Information System (INIS)
Amusia, M.Ya.; Sheftel, S.I.
1976-01-01
The photoionization cross section of 4d 10 subshell of La atom is calculated. The cross section curve near its threshold is strongly modified by rearrangement of outer shells in the process of photoionization. (Auth.)
Synchrotron Photoionization Investigation of the Oxidation of Ethyl tert-Butyl Ether.
Winfough, Matthew; Yao, Rong; Ng, Martin; Catani, Katherine; Meloni, Giovanni
2017-02-23
The oxidation of ethyl tert-butyl ether (ETBE), a widely used fuel oxygenated additive, is investigated using Cl atoms as initiators in the presence of oxygen. The reaction is carried out at 293, 550, and 700 K. Reaction products are probed by a multiplexed chemical kinetics photoionization mass spectrometer coupled with the synchrotron radiation produced at the Advanced Light Source (ALS) of the Lawrence Berkeley National Laboratory. Products are identified on the basis of mass-to-charge ratio, ionization energies, and shape of photoionization spectra. Reaction pathways are proposed together with detected primary products.
THE DISK-WIND-JET CONNECTION IN THE BLACK HOLE H 1743-322
Energy Technology Data Exchange (ETDEWEB)
Miller, J. M.; King, A. L. [Department of Astronomy, University of Michigan, 500 Church Street, Ann Arbor, MI 48109-1042 (United States); Raymond, J. [Smithsonian Astrophysical Observatory, 60 Garden Street, Cambridge, MA 02138 (United States); Fabian, A. C. [Institute of Astronomy, University of Cambridge, Madingley Road, Cambridge CB3 OHA (United Kingdom); Reynolds, C. S. [Department of Astronomy, University of Maryland, College Park, MD 20742 (United States); Kallman, T. R. [Laboratory for High Energy Astrophysics, NASA Goddard Space Flight Center, Code 662, Greenbelt, MD 20771 (United States); Cackett, E. M. [Department of Physics and Astronomy, Wayne State University, 666 West Hancock Street, Detroit, MI 48201 (United States); Van der Klis, M. [Astronomical Institute ' Anton Pannekoek' , University of Amsterdam, Science Park 904, 1098-XH, Amsterdam (Netherlands); Steeghs, D. T. H., E-mail: jonmm@umich.edu [Department of Physics, University of Warwick, Coventry CV4 7AL (United Kingdom)
2012-11-01
X-ray disk winds are detected in spectrally soft, disk-dominated phases of stellar-mass black hole outbursts. In contrast, compact, steady, relativistic jets are detected in spectrally hard states that are dominated by non-thermal X-ray emission. Although these distinctive outflows appear to be almost mutually exclusive, it is possible that a disk wind persists in hard states but cannot be detected via X-ray absorption lines owing to very high ionization. Here, we present an analysis of a deep, 60 ks Chandra/HETGS observation of the black hole candidate H 1743-322 in the low/hard state. The spectrum shows no evidence of a disk wind, with tight limits, and within the range of ionizing flux levels that were measured in prior Chandra observations wherein a wind was clearly detected. In H 1743-322, at least, disk winds are actually diminished in the low/hard state, and disk winds and jets are likely state dependent and anti-correlated. These results suggest that although the launching radii of winds and jets may differ by orders of magnitude, they may both be tied to a fundamental property of the inner accretion flow, such as the mass accretion rate and/or the magnetic field topology of the disk. We discuss these results in the context of disk winds and jets in other stellar-mass black holes, and possible launching mechanisms for black hole outflows.
ANALYTIC FITS FOR PARTIAL PHOTOIONIZATION CROSS-SECTIONS
VERNER, DA; YAKOVLEV, DG
We present a compact, uniform and complete set of analytic fits to the partial Hartree-Dirac-Slater photoionization cross sections for the ground state shells of all atoms and ions of elements from H to Zn (Z less-than-or-equal-to 30). Comparison with experiment and theory demonstrates generally
International Nuclear Information System (INIS)
Jian-Hua, Wu; Jian-Min, Yuan
2009-01-01
Interference effects on the photoionization cross sections between two neighbouring atoms are considered based on the coherent scattering of the ionized electrons by the two nuclei when their separation is less than or comparable to the de Broglie wave length of the ionized electrons. As an example, the single atomic nitrogen ionization cross section and the total cross sections of two nitrogen atoms with coherently added photoionization amplitudes are calculated from the threshold to about 60 Å (1 Å = 0.1 nm) of the photon energy. The photoionization cross sections of atomic nitrogen are obtained by using the close-coupling R-matrix method. In the calculation 19 states are included. The ionization energy of the atomic nitrogen and the photoionization cross sections agree well with the experimental results. Based on the R-matrix results of atomic nitrogen, the interference effects between two neighbouring nitrogen atoms are obtained. It is shown that the interference effects are considerable when electrons are ionized just above the threshold, even for the separations between the two atoms are larger than two times of the bond length of N 2 molecules. Therefore, in hot and dense samples, effects caused by the coherent interference between the neighbours are expected to be observable for the total photoionization cross sections. (atomic and molecular physics)
The enigmatic wind of 55 Cygni
Czech Academy of Sciences Publication Activity Database
Haucke, M.; Kraus, Michaela; Venero, R.O.J.; Cidale, L.S.; Nickeler, Dieter Horst; Tomić, S.; Curé, M.
2013-01-01
Roč. 56, č. 1 (2013), s. 191-194 E-ISSN 1669-9521 R&D Projects: GA ČR(CZ) GAP209/11/1198 Institutional support: RVO:67985815 Keywords : line profiles * stellar wind * spectroscopic observin Subject RIV: BN - Astronomy, Celestial Mechanics, Astrophysics http://www. astronomia argentina.org.ar/b56/2013baaa...56...191H.pdf
Interaction of mass-loaded solar wind flow with blunt body
International Nuclear Information System (INIS)
Breus, T.K.; Krymskii, A.M.; Mitnitskii, V.Ya.
1987-01-01
The aim of this paper is the numerical modeling of the solar wind interaction with Venus taking into account the mass loading effect due to the photoionization of the Venus neutral oxygen corona. The analysis has shown that this effect unambiguously explains the number of peculiarities of the SW-Venus interaction pattern that could not be quantitatively explained before, namely the shock front position, and the characteristics of the SW flow and magnetic field in the Venus ionosheath observed from experiments onboard of Venera-9 and -10 and Pioneer-Venus spacecraft. (author)
Electron Interference in Molecular Circular Polarization Attosecond XUV Photoionization
Directory of Open Access Journals (Sweden)
Kai-Jun Yuan
2015-01-01
Full Text Available Two-center electron interference in molecular attosecond photoionization processes is investigated from numerical solutions of time-dependent Schrödinger equations. Both symmetric H\\(_2^+\\ and nonsymmetric HHe\\(^{2+}\\ one electron diatomic systems are ionized by intense attosecond circularly polarized XUV laser pulses. Photoionization of these molecular ions shows signature of interference with double peaks (minima in molecular attosecond photoelectron energy spectra (MAPES at critical angles \\(\\vartheta_c\\ between the molecular \\(\\textbf{R}\\ axis and the photoelectron momentum \\(\\textbf{p}\\. The interferences are shown to be a function of the symmetry of electronic states and the interference patterns are sensitive to the molecular orientation and pulse polarization. Such sensitivity offers possibility for imaging of molecular structure and orbitals.
Polarized bow shocks reveal features of the winds and environments of massive stars
Shrestha, Manisha
2018-01-01
Massive stars strongly affect their surroundings through their energetic stellar winds and deaths as supernovae. The bow shock structures created by fast-moving massive stars contain important information about the winds and ultimate fates of these stars as well as their local interstellar medium (ISM). Since bow shocks are aspherical, the light scattered in the dense shock material becomes polarized. Analyzing this polarization reveals details of the bow shock geometry as well as the composition, velocity, density, and albedo of the scattering material. With these quantities, we can constrain the properties of the stellar wind and thus the evolutionary state of the star, as well as the dust composition of the local ISM.In my dissertation research, I use a Monte Carlo radiative transfer code that I optimized to simulate the polarization signatures produced by both resolved and unresolved stellar wind bow shocks (SWBS) illuminated by a central star and by shock emission. I derive bow shock shapes and densities from published analytical calculations and smooth particle hydrodynamic (SPH) models. In the case of the analytical SWBS and electron scattering, I find that higher optical depths produce higher polarization and position angle rotations at specific viewing angles compared to theoretical predictions for low optical depths. This is due to the geometrical properties of the bow shock combined with multiple scattering effects. For dust scattering, the polarization signature is strongly affected by wavelength, dust grain properties, and viewing angle. The behavior of the polarization as a function of wavelength in these cases can distinguish among different dust models for the local ISM. In the case of SPH density structures, I investigate how the polarization changes as a function of the evolutionary phase of the SWBS. My dissertation compares these simulations with polarization data from Betelgeuse and other massive stars with bow shocks. I discuss the
Luminosity excesses in low-mass young stellar objects - a statistical study
International Nuclear Information System (INIS)
Strom, K.M.; Strom, S.E.; Kenyon, S.J.; Hartmann, L.
1988-01-01
This paper presents a statistical study in which the observed total luminosity is compared quantitatively with an estimate of the stellar luminosity for a sample of 59 low-mass young stellar objects (YSOs) in the Taurus-Auriga complex. In 13 of the analyzed YSOs, luminosity excesses greater than 0.20 are observed together with greater than 0.6 IR excesses, which typically contribute the bulk of the observed excess luminosity and are characterized by spectral energy distributions which are flat or rise toward long wavelengths. The analysis suggests that YSOs showing the largest luminosity excesses typically power optical jets and/or molecular outflows or have strong winds, as evidenced by the presence of O I emission, indicating a possible correlation between accretion and mass-outflow properties. 38 references
The effect of mass loss by stellar wind on the chemical enrichment of the galaxy
International Nuclear Information System (INIS)
Chiosi, C.
1979-01-01
The rate of production of heavy elements is rediscussed using the models of Arnett (1978) for late stage nucleosynthesis in massive stars, the M(M,) relationship of Chiosi et al. (1978b) for losing mass models in the core H and He-Burning phases, and the stellar birth rate of Miller and Scalo (1978). Contrary to that found by Wheeler et al (1978), we do not encounter the difficulty of heavy element overproduction. The explosive nucleosynthesis from massive stars is still compatible with the observed abundance distribution of the solar system, and a stellar birth rate decreasing over the history of the galactic disk. (orig.)
Stellar Interlopers Caught Speeding Through Space
2009-01-01
[figure removed for brevity, see original site] [figure removed for brevity, see original site] [figure removed for brevity, see original site] [figure removed for brevity, see original site] Figure 1 Figure 2 Figure 3 Figure 4 Click on individual image for larger view Resembling comets streaking across the sky, these four speedy stars are plowing through regions of dense interstellar gas and creating brilliant arrowhead structures and trailing tails of glowing gas. These bright arrowheads, or bow shocks, can be seen in these four images taken with NASA's Hubble Space Telescope. The bow shocks form when the stars' powerful stellar winds, streams of matter flowing from the stars, slam into surrounding dense gas. The phenomenon is similar to that seen when a speeding boat pushes through water on a lake. The stars in these images are among 13 runaway stars spotted by Hubble's Advanced Camera for Surveys. The stars appear to be young, just millions of years old. Their ages are based on their colors and the presence of strong stellar winds, a signature of youthful stars. Depending on their distance from Earth, the bullet-nosed bow shocks could be 100 billion to a trillion miles wide (the equivalent of 17 to 170 solar system diameters, measured out to Neptune's orbit). The bow shocks indicate that the stars are moving fast, more than 180,000 kilometers an hour (more than 112,000 miles an hour) with respect to the dense gas they are plowing through. They are traveling roughly five times faster than typical young stars, relative to their surroundings. The high-speed stars have traveled far from their birth places. Assuming their youthful phase lasts only a million years and they are moving at roughly 180,000 kilometers an hour, the stars have journeyed 160 light-years. The Hubble observations were taken between October 2005 and July 2006.
Metallic Winds in Dwarf Galaxies
International Nuclear Information System (INIS)
Robles-Valdez, F.; Rodríguez-González, A.; Hernández-Martínez, L.; Esquivel, A.
2017-01-01
We present results from models of galactic winds driven by energy injected from nuclear (at the galactic center) and non-nuclear starbursts. The total energy of the starburst is provided by very massive young stellar clusters, which can push the galactic interstellar medium and produce an important outflow. Such outflow can be a well or partially mixed wind, or a highly metallic wind. We have performed adiabatic 3D N -Body/Smooth Particle Hydrodynamics simulations of galactic winds using the gadget-2 code. The numerical models cover a wide range of parameters, varying the galaxy concentration index, gas fraction of the galactic disk, and radial distance of the starburst. We show that an off-center starburst in dwarf galaxies is the most effective mechanism to produce a significant loss of metals (material from the starburst itself). At the same time, a non-nuclear starburst produces a high efficiency of metal loss, in spite of having a moderate to low mass loss rate.
Role of Turbulent Damping in Cosmic Ray Galactic Winds
Holguin, Francisco; Ruszkowski, Mateusz; Lazarian, Alex; Yang, H. Y. Karen
2018-06-01
Large-scale galactic winds driven by stellar feedback are one phenomenon that influences the dynamical and chemical evolution of a galaxy, pushing and redistributing material throughout the interstellar medium (ISM) and galactic halo. A detailed understanding of the exact physical mechanisms responsible for these winds is lacking. Non-thermal feedback from galactic cosmic rays (CR), high-energy charged particles accelerated in supernovae and young stars, can impact the efficiency in accelerating the wind. In the self-confinement model, CR stream along magnetic field lines at the Alfven speed due to scattering off self-excited Aflv{é}n waves. However, magneto-hydrodynamic (MHD) turbulence stirred up by stellar feedback dissipates these confining waves, allowing CR to be super Aflvenic. Previous simulations relying on a simplified model of transport have shown that super-Alfv{é}nic streaming of CRs can launch a stronger wind. We perform three-dimensional MHD simulations of a section of a galactic disk, including CR streaming dependent on the local environment, using a realistic model of turbulent dissipation of Alfven waves presented in Lazarian (2016). In this implementation, the CR streaming speed can be super Alfv{é}nic depending on local conditions. We compare results for Alfv{é}nic and locally determined streaming, and find that gas/CR distributions and instantaneous mass loading factor of the wind are different depending on the level of turbulence.Lazarian, A. “Damping of Alfven waves by turbulence and its consequences: from cosmic-ray streaming to launching winds.” ApJ. Vol. 833, Num. 2. (2016).
Banerjee, Sambaran
2018-01-01
The study of stellar-remnant black holes (BH) in dense stellar clusters is now in the spotlight, especially due to their intrinsic ability to form binary black holes (BBH) through dynamical encounters, which potentially coalesce via gravitational-wave (GW) radiation. In this work, which is a continuation from a recent study (Paper I), additional models of compact stellar clusters with initial masses ≲ 105 M⊙ and also those with small fractions of primordial binaries (≲ 10 per cent) are evolved for long term, applying the direct N-body approach, assuming state-of-the-art stellar-wind and remnant-formation prescriptions. That way, a substantially broader range of computed models than that in Paper I is achieved. As in Paper I, the general-relativistic BBH mergers continue to be mostly mediated by triples that are bound to the clusters rather than happen among the ejected BBHs. In fact, the number of such in situ BBH mergers, per cluster, tends to increase significantly with the introduction of a small population of primordial binaries. Despite the presence of massive primordial binaries, the merging BBHs, especially the in situ ones, are found to be exclusively dynamically assembled and hence would be spin-orbit misaligned. The BBHs typically traverse through both the LISA's and the LIGO's detection bands, being audible to both instruments. The 'dynamical heating' of the BHs keeps the electron-capture-supernova (ECS) neutron stars (NS) from effectively mass segregating and participating in exchange interactions; the dynamically active BHs would also exchange into any NS binary within ≲1 Gyr. Such young massive and open clusters have the potential to contribute to the dynamical BBH merger detection rate to a similar extent as their more massive globular-cluster counterparts.
International Nuclear Information System (INIS)
Mandal, P.K.; Seema, A.U.; Das, R.C.; Shah, M.L.; Dev, Vas; Suri, B.M.
2013-01-01
Three-colour three-step photoionization spectroscopy of uranium has been performed in a U-Ne hollow cathode discharge tube by temporally resolving three-colour photoionization optogalvanic (PIOG) signal from the normal optogalvanic (OG) signal using three tunable pulsed dye lasers. U-Ne hollow cathode discharge tube has been used as a source of uranium atomic vapour and photoionization detector. Using this technique, photoionization spectra of uranium have been investigated systematically in the energy region 52150-52590 cm -1 , through three different excitation pathways, originating from its ground state, 0 cm -1 ( 5 L 0 6 ). By analyzing the three-colour photoionization spectra sixty new even-parity autoionization resonances of uranium have been identified and their probable total angular momentum (J) values have been assigned according to the J-momentum selection rule. (author)
Winds of AGB stars: does size matter?
International Nuclear Information System (INIS)
Hoefner, S
2008-01-01
Asymptotic giant branch (AGB) stars are showing clear signs of significant mass loss through cool stellar winds. These outflows are attributed to the combined effects of pulsation-induced shocks and radiation pressure on dust grains formed in the outer atmospheric layers. This paper gives an overview of the current status of radiation-hydrodynamical modelling of these processes, and presents a toy model that allows analysis of certain features of detailed models, such as the influence of grain size dependent opacities and basic differences in winds of C- and M-type AGB stars.
International Nuclear Information System (INIS)
Schwell, Martin; Bénilan, Yves; Fray, Nicolas; Gazeau, Marie-Claire; Es-Sebbar, Et.; Garcia, Gustavo A.; Nahon, Laurent; Champion, Norbert; Leach, Sydney
2012-01-01
Highlights: ► We study the VUV photoionization of acetamide in the 8–24 eV photon energy range. ► Electron/ion coincidence measurements are performed using synchrotron radiation. ► The adiabatic ionization energy of acetamide is determined by TPEPICO measurements. ► VUV induced fragmentation pathways of acetamide are assigned and discussed. - Abstract: A VUV photoionization study of acetamide was carried out over the 8–24 eV photon energy range using synchrotron radiation and photoelectron/photoion coincidence (PEPICO) spectroscopy. Threshold photoelectron photoion coincidence (TPEPICO) measurements were also made. Photoion yield curves and branching ratios were measured for the parent ion and six fragment ions. The adiabatic ionization energy of acetamide was determined as I.E. (1 2 A′) = (9.71 ± 0.02) eV, in agreement with an earlier reported photoionization mass spectrometry (PIMS) value. The adiabatic energy of the first excited state of the ion, 1 2 A″, was determined to be ≈10.1 eV. Assignments of the fragment ions and the pathways of their formation by dissociative photoionization were made. The neutral species lost in the principal dissociative photoionization processes are CH 3 , NH 2 , NH 3 , CO, HCCO and NH 2 CO. Heats of formation are derived for all ions detected and are compared with literature values. Some astrophysical implications of these results are discussed.
Intershell correlations in photoionization of outer shells
Energy Technology Data Exchange (ETDEWEB)
Amusia, M.Ya. [The Racah Institute of Physics, The Hebrew University of Jerusalem, Jerusalem 91904 (Israel); A.F. Ioffe Physical-Technical Institute, St. Petersburg 194021 (Russian Federation); Chernysheva, L.V. [A.F. Ioffe Physical-Technical Institute, St. Petersburg 194021 (Russian Federation); Drukarev, E.G. [National Research Center “Kurchatov Institute”, Konstantinov Petersburg Nuclear Physics Institute, St. Petersburg 188300 (Russian Federation)
2016-02-15
We demonstrate that the cross sections for photoionization of the outer shells are noticeably modified at the photon energies close to the thresholds of ionization of the inner shells due to correlations with the latter. The correlations may lead to increase or to decrease of the cross sections just above the ionization thresholds.
Intershell correlations in photoionization of outer shells
International Nuclear Information System (INIS)
Amusia, M.Ya.; Chernysheva, L.V.; Drukarev, E.G.
2016-01-01
We demonstrate that the cross sections for photoionization of the outer shells are noticeably modified at the photon energies close to the thresholds of ionization of the inner shells due to correlations with the latter. The correlations may lead to increase or to decrease of the cross sections just above the ionization thresholds.
Continuum multiple-scattering approach to electron-molecule scattering and molecular photoionization
International Nuclear Information System (INIS)
Dehmer, J.L.; Dill, D.
1979-01-01
The multiple-scattering approach to the electronic continuum of molecules is described. The continuum multiple-scattering model (CMSM) was developed as a survey tool and, as such was required to satisfy two requirements. First, it had to have a very broad scope, which means (i) molecules of arbitrary geometry and complexity containing any atom in the periodic system, (ii) continuum electron energies from 0-1000 eV, and (iii) capability to treat a large range of processes involving both photoionization and electron scattering. Second, the structure of the theory was required to lend itself to transparent, physical interpretation of major spectral features such as shape resonances. A comprehensive theoretical framework for the continuum multiple scattering method is presented, as well as its applications to electron-molecule scattering and molecular photoionization. Highlights of recent applications in these two areas are reviewed. The major impact of the resulting studies over the last few years has been to establish the importance of shape resonances in electron collisions and photoionization of practically all (non-hydride) molecules
Photoionization cross sections: present status and future needs
International Nuclear Information System (INIS)
Manson, S.T.
1988-01-01
The existing experimental data situation for photoionization cross section of ground-state atoms, excited states and positive ions is reviewed. The ability of theory to predict these cross sections is also discussed. The likely progress for the near future is presented [pt
International Nuclear Information System (INIS)
Clark, R.E.H.; Cowan, R.D.; Bobrowicz, F.W.
1986-01-01
Hartree--Fock wave functions have been used to calculate configuration -averaged photoionization cross sections and ionization energies for orbitals 1s< or =nl< or =5g in He-like through Al-like isoelectroni csequences. The photoionization cross sections have been fitted as a function of the nuclear charge, Z, and photon energy, X, in threshold units, with average error of less than 10%. The ionization energies have been fitted as a function of Z with errors of less than 0.5%
International Nuclear Information System (INIS)
Masuoka, Toshio; Kobayashi, Ataru
2004-01-01
Single- and double-photoionization processes of nitrogen dioxide (NO 2 ) have been studied in the photon energy region of 37-125 eV by use of time-of-flight mass spectrometry and the photoion-photoion coincidence method together with synchrotron radiation. The single- and double-photoionization cross-sections of NO 2 are determined. Ion branching ratios and the partial cross-sections for the individual ions, respectively, produced from the parent NO 2 + and NO 2 2+ ions are also determined separately at excitation energies where the molecular and dissociative single- and double-photoionization processes occur simultaneously. It was found that dissociation of the parent ions is dominant both in single and double photoionization. The thresholds for the O + + NO + and N + + O + dissociation channels of NO 2 2+ are at 35.0 ± 0.3 and 43.6 ± 0.3 eV, respectively. Kinetic energy releases in these two dissociation channels of NO 2 2+ have also been elucidated
Stokes polarimetry of main-line OH emission from stellar masers
International Nuclear Information System (INIS)
Claussen, M.J.; Fix, J.D.
1982-01-01
Main-line OH emission has been measured in all four Stokes parameters from seven late-type variable stars and the F8 supergiant IRC+10420. Linearly polarized features were detected in UX Cyg, U Ori, and IRC+10420 at 1665 MHz. The linearly polarized features in UX Cyg and IRC +10420, when combined with adjacent circularly polarized features suggest Zeeman patterns. A polarization pattern in IRC+10420 is probably the best example of a complete Zeeman pattern yet observed in stellar masers, although it appears to lack the shifted linear (sigma) components. This study, combined with other recent work, shows that linearly polarized features in stellar sources are uncommon. Only about 10% of the stellar OH sources show linearly polarized features. As an aid in accounting for the observed polarization properties of stellar OH masers, model mass flows were calculated using magnetic field structures similar to that of the solar wind. Conclusions drawn from this model were: (1) unpolarized or weakly circularly polarized emission from sources can arise from the entire circumstellar shell; (2) circular polarization without linear polarization can be produced either by emission from the entire shell or by enhanced OH densities in small regions of the shell provided there are sufficient free electrons present to depolarize the linear components; and (3) Zeeman patterns which include both circular and linear polarizations can be produced in OH density enhancements if electron densities are low. The electron densities required for effective Faraday depolarization yield emission measures of the order of 10 9 pc cm -6 . Given the large distances of stellar OH masers, the thermal continuum emission from such depolarizing electrons would probably be undetectable
X-ray emission lines from photoionized plasmas
International Nuclear Information System (INIS)
Liedahl, D.A.
1992-11-01
Plasma emission codes have become a standard tool for the analysis of spectroscopic data from cosmic X-ray sources. However, the assumption of collisional equilibrium, typically invoked in these codes, renders them inapplicable to many important astrophysical situations, particularly those involving X-ray photoionized nebulae, which are likely to exist in the circumsource environments of compact X-ray sources. X-ray line production in a photoionized plasma is primarily the result of radiative cascades following recombination. Through the development of atomic models of several highly-charged ions, this work extends the range of applicability of discrete spectral models to plasmas dominated by recombination. Assuming that ambient plasma conditions lie in the temperature range 10 5 --10 6 K and the density range 10 11 --10 16 cm -3 , X-ray line spectra are calculated over the wavelength range 5--45 angstrom using the HULLAC atomic physics package. Most of the work focuses on the Fe L-shell ions. Line ratios of the form (3s-2p)/(3d-2p) are shown to characterize the principal mode of line excitation, thereby providing a simple signature of photoionization. At electron densities exceeding 10 12 cm -3 , metastable state populations in the ground configurations approach their LTE value, resulting in the enrichment of the Fe L-shell recombination spectrum and a set of density-sensitive X-ray line ratios. Radiative recombination continua and emission lines produced selectively by Δn = 0 dielectronic recombination are shown to provide two classes of temperature diagnostics. Because of the extreme overionization, the recombination continua are expected to be narrow (ΔE/E much-lt 1), with ΔE = kT. Dielectronic recombination selectively drives radiative transitions that originate on states with vacancies in the 2s subshell, states that are inaccessible under pure RR population kinetics
NIST Photoionization of CO2 (ARPES) Database
SRD 119 NIST Photoionization of CO2 (ARPES) Database (Web, free access) CO2 is studied using dispersed synchrotron radiation in the 650 Å to 850 Å spectral region. The vibrationally resolved photoelectron spectra are analyzed to generate relative vibrational transition amplitudes and the angular asymmetry parameters describing the various transitions observed.
Vacuum ultraviolet photoionization mass spectrometric study of cyclohexene.
Chen, Jun; Cao, Maoqi; Wei, Bin; Ding, Mengmeng; Shan, Xiaobin; Liu, Fuyi; Sheng, Liusi
2016-02-01
In this work, photoionization and dissociation of cyclohexene have been studied by means of coupling a reflectron time-of-flight mass spectrometer with the tunable vacuum ultraviolet (VUV) synchrotron radiation. The adiabatic ionization energy of cyclohexene as well as the appearance energies of its fragment ions C6 H9 (+) , C6 H7 (+) , C5 H7 (+) , C5 H5 (+) , C4 H6 (+) , C4 H5 (+) , C3 H5 (+) and C3 H3 (+) were derived from the onset of the photoionization efficiency (PIE) curves. The optimized structures for the transition states and intermediates on the ground state potential energy surfaces related to photodissociation of cyclohexene were characterized at the ωB97X-D/6-31+g(d,p) level. The coupled cluster method, CCSD(T)/cc-pVTZ, was employed to calculate the corresponding energies with the zero-point energy corrections by the ωB97X-D/6-31+g(d,p) approach. Combining experimental and theoretical results, possible formation pathways of the fragment ions were proposed and discussed in detail. The retro-Cope rearrangement was found to play a crucial role in the formation of C4 H6 (+) , C4 H5 (+) and C3 H5 (+) . Intramolecular hydrogen migrations were observed as dominant processes in most of the fragmentation pathways of cyclohexene. The present research provides a clear picture of the photoionization and dissociation processes of cyclohexene in the 8- to 15.5-eV photon energy region. Copyright © 2016 John Wiley & Sons, Ltd.
Dorodnitsyn, Anton V.; Kallman, Timothy R.
2012-01-01
We present calculations of active galactic nucleus winds at approx.parsec scales along with the associated obscuration. We take into account the pressure of infrared radiation on dust grains and the interaction of X-rays from a central black hole with hot and cold plasma. Infrared radiation (IR) is incorporated in radiation-hydrodynamic simulations adopting the flux-limited diffusion approximation. We find that in the range of X-ray luminosities L = 0.05-0.6 L(sub Edd), the Compton-thick part of the flow (aka torus) has an opening angle of approximately 72deg - 75deg regardless of the luminosity. At L > or approx. 0.1, the outflowing dusty wind provides the obscuration with IR pressure playing a major role. The global flow consists of two phases: the cold flow at inclinations (theta) > or approx.70deg and a hot, ionized wind of lower density at lower inclinations. The dynamical pressure of the hot wind is important in shaping the denser IR-supported flow. At luminosities < or = 0.1 L(sub Edd) episodes of outflow are followed by extended periods when the wind switches to slow accretion. Key words: acceleration of particles . galaxies: active . hydrodynamics . methods: numerical Online-only material: color figures
International Nuclear Information System (INIS)
Jaenkaelae, K.; Alagia, M.; Feyer, V.; Richter, R.; Prince, K. C.
2011-01-01
Laser orientation in the initial state has been used to study the properties of satellite transitions in inner-shell photoionization of rubidium atoms. The linear magnetic dichroism in the angular distribution (LMDAD) has been utilized to probe the continuum waves of orbital angular momentum conserving monopole, and angular momentum changing conjugate satellites, accompanying the 4p ionization of atomic Rb. We show experimentally that LMDAD of both types of satellite transitions is nonzero and that LMDAD of monopole satellites, measured as a function of photon energy, mimics the LMDAD of direct photoionization, whereas the LMDAD of conjugate transitions deviates drastically from that trend. The results indicate that conjugate transitions cannot be described theoretically without explicit inclusion of electron-electron interaction. The present data can thus be used as a very precise test of current models for photoionization.
Gao, Hong
The tunable vacuum ultraviolet (VUV) laser generated through the two-photon resonance-enhanced four-wave mixing scheme is combined with the newly developed time-slice velocity map imaging photoion method to study the photodissociation of small molecules in the VUV region, and with the velocity map imaging photoelectron method to study the photoionization of free radicals. The photodissociation dynamics of NO in the energy region around 13.5 eV has been investigated. Branching ratios of the three lowest dissociation channels of 12C 16O that produce C(3P) + O(3P), C( 1D) + O(3P) and C(3P) + O(1D) are measured for the first time in the VUV region from 102,500 cm-1 to 110,500 cm-1, valuable information of the dissociation dynamics for this prototype system has been deduced. We demonstrated an experiment that has two independently tunable VUV lasers and a time-slice velocity map imaging setup, this provides us a global way to perform systematic state-selected photodissociation of small molecules via state-selected detection of the atomic products in the VUV region. The velocity map imaging photoelectron method was successfully used to obtain the photoelectron spectrum of the propargyl radical (C3H3) via a single VUV photoionization process. The propargyl radical is generated by the 193 nm laser photodissociation of the precursor C3H3Cl. This is the first time that the velocity map imaging photoelectron method is used to get the photoelectron spectra of free radicals, indicating that it is a powerful technique for studying the photoionization of free radicals which are always hard to be produced with high enough number densities for spectroscopic studies. This dissertation is mainly based on the following peer-reviewed journal articles: 1. Hong Gao, Yang Pan, Lei Yang, Jingang Zhou, C. Y. Ng and William M. Jackson. "Time-slice velocity-map ion imaging studies of the Photodissociation of NO in the vacuum ultraviolet region", the Journal of Chemical Physics, 136, 134302
International Nuclear Information System (INIS)
Silfvast, W.T.; Wood, O.R. II; Al-Salameh, D.Y.
1986-01-01
The two-electron (shake-up) photoionization process has been shown to be an effective mechanism for producing large population inversions in He/sup +/ with gain at 164 nm and in Ar/sup +/ with gain at 428 and 477 nm and for observing the first autoionizing states in Cd/sup +/. Such a mechanism was recently proposed as an excitation mechanism for a VUV laser in lithium. In each species the rapid excitation and detection using broadband emission from a 30-mJ 100-ps duration laser-produced plasma and a detection system with subnanosecond time resolution were essential in observing these effects. In He, gains of up to 0.8 cm/sup -1/ for durations of 2-4 ns at 164.0 nm on the He-like (n = 3-2) transition in He/sup +/ were measured by comparing the plasma emission from a well-defined volume with and without the presence of a mirror of known reflectivity. The n = 3 upper laser level is pumped not only directly via two-electron photoionization from the neutral ground state but also indirectly (in times of the order of 1-2 ns) via electron collisions from photoionization-pumped higher-lying levels. The decay rate of the photoionization-pumped radiation-trapped lower laser level is increased by a unique process involving absorption of radiation via photoionization of ground state neutral helium atoms
THE DISK-WIND-JET CONNECTION IN THE BLACK HOLE H 1743–322
International Nuclear Information System (INIS)
Miller, J. M.; King, A. L.; Raymond, J.; Fabian, A. C.; Reynolds, C. S.; Kallman, T. R.; Cackett, E. M.; Van der Klis, M.; Steeghs, D. T. H.
2012-01-01
X-ray disk winds are detected in spectrally soft, disk-dominated phases of stellar-mass black hole outbursts. In contrast, compact, steady, relativistic jets are detected in spectrally hard states that are dominated by non-thermal X-ray emission. Although these distinctive outflows appear to be almost mutually exclusive, it is possible that a disk wind persists in hard states but cannot be detected via X-ray absorption lines owing to very high ionization. Here, we present an analysis of a deep, 60 ks Chandra/HETGS observation of the black hole candidate H 1743–322 in the low/hard state. The spectrum shows no evidence of a disk wind, with tight limits, and within the range of ionizing flux levels that were measured in prior Chandra observations wherein a wind was clearly detected. In H 1743–322, at least, disk winds are actually diminished in the low/hard state, and disk winds and jets are likely state dependent and anti-correlated. These results suggest that although the launching radii of winds and jets may differ by orders of magnitude, they may both be tied to a fundamental property of the inner accretion flow, such as the mass accretion rate and/or the magnetic field topology of the disk. We discuss these results in the context of disk winds and jets in other stellar-mass black holes, and possible launching mechanisms for black hole outflows.
Photoionization of cobalt impuritiesin zinc oxide
Czech Academy of Sciences Publication Activity Database
Ivanov, V.; Godlewski, M.; Dejneka, Alexandr
2015-01-01
Roč. 252, č. 9 (2015), s. 1988-1992 ISSN 0370-1972 R&D Projects: GA MŠk(CZ) LM2011029; GA ČR GAP108/12/1941 Grant - others:SAFMAT(XE) CZ.2.16/3.1.00/22132 Institutional support: RVO:68378271 Keywords : absorption band * cobalt * photoionization * electron spin resonance * pulsed mode * ZnO Subject RIV: BM - Solid Matter Physics ; Magnetism Impact factor: 1.522, year: 2015
Metastable decay of photoionized niobium clusters: Evaporation vs fission fragmentation
International Nuclear Information System (INIS)
Cole, S.K.; Liu, K.; Riley, S.J.
1986-01-01
The metastable decay of photoionized niobium clusters (Nb/sub n/ + ) has been observed in a newly constructed cluster beam machine. The decay manifests itself in the time-of-flight (TOF) mass spectrum as an asymmetric broadening of daughter ion peaks. Pulsed ion extraction has been used to measure the decay rate constants and to establish the mechanism of the fragmentation, evaporation and/or fission of the photoionized clusters. It is found that within the experimental time window evaporation dominates for the smaller clusters (n 6 sec -1 . The average kinetic energy release is also determined and is found to be on the order of 5 MeV. 8 refs., 3 figs., 1 tab
Extended fine structure in the K-shell photoionization spectrum of Br2
International Nuclear Information System (INIS)
Dill, D.; Dehmer, J.L.
1975-01-01
The multiple-scattering approach to molecular wavefunctions in the electronic continuum has been used recently to elucidate the structure of the shape resonance just above threshold in the K-shell photoionization spectrum of N 2 . A similar calculation for Br 2 has yielded significantly different results, i.e., there is no shape resonance; appearing instead is a single resonance in the discrete spectrum, and the photoionization spectrum is found to oscillate with appreciable amplitude throughout the spectral range investigated, from threshold to 60 Ry
Energy Technology Data Exchange (ETDEWEB)
Finley, Adam J.; Matt, Sean P., E-mail: af472@exeter.ac.uk [University of Exeter (UK), Department of Physics and Astronomy, Stoker Road, Devon, Exeter, EX4 4QL (United Kingdom)
2017-08-10
Cool stars with outer convective envelopes are observed to have magnetic fields with a variety of geometries, which on large scales are dominated by a combination of the lowest-order fields such as the dipole, quadrupole, and octupole modes. Magnetized stellar wind outflows are primarily responsible for the loss of angular momentum from these objects during the main sequence. Previous works have shown the reduced effectiveness of the stellar wind braking mechanism with increasingly complex but singular magnetic field geometries. In this paper, we quantify the impact of mixed dipolar and quadrupolar fields on the spin-down torque using 50 MHD simulations with mixed fields, along with 10 each of the pure geometries. The simulated winds include a wide range of magnetic field strength and reside in the slow-rotator regime. We find that the stellar wind braking torque from our combined geometry cases is well described by a broken power-law behavior, where the torque scaling with field strength can be predicted by the dipole component alone or the quadrupolar scaling utilizing the total field strength. The simulation results can be scaled and apply to all main-sequence cool stars. For solar parameters, the lowest-order component of the field (dipole in this paper) is the most significant in determining the angular momentum loss.
Role of ionization fronts in the colliding wind model of planetary nebulae
International Nuclear Information System (INIS)
Giuliani, J.L. Jr.
1981-01-01
A similarity transformation is used to study the expansion of a planetary nebula which is driven by a fast stellar wind as well as an expanding H II region. The undisturbed gas is taken to be the remnant of a slow, red giant wind. The present analysis improves upon Kwok, Purton, and FitzGerald's colliding wind model for the formation of planetary nebulae since it includes the dynamical influence of ionization fronts, and calculates the variation of velocity and density within the flow
Recoil momenta distributions in the double photoionization
International Nuclear Information System (INIS)
Amusia, M Ya; Liverts, E Z; Drukarev, E G; Mikhai, A I
2014-01-01
We calculate the distributions in recoil momenta for the high energy double photoionization of helium caused by quasifree mechanism. The distributions obtain local maxima at small values of the recoil momenta. This agrees with earlier predictions and recent experimental data. Angular correlations which reach the largest value for 'back-to-back' configuration of photoelectrons are also obtained.
Velasco, A M; Lavín, C; Dolgounitcheva, O; Ortiz, J V
2014-08-21
Vertical excitation energies of the methyl and silyl radicals were inferred from ab initio electron propagator calculations on the electron affinities of CH3(+) and SiH3(+). Photoionization cross sections and angular distribution of photoelectrons for the outermost orbitals of both CH3 and SiH3 radicals have been obtained with the Molecular Quantum Defect Orbital method. The individual ionization cross sections corresponding to the Rydberg channels to which the excitation of the ground state's outermost electron gives rise are reported. Despite the relevance of methyl radical in atmospheric chemistry and combustion processes, only data for the photon energy range of 10-11 eV seem to be available. Good agreement has been found with experiment for photoionization cross section of this radical. To our knowledge, predictions of the above mentioned photoionization parameters on silyl radical are made here for the first time, and we are not aware of any reported experimental measurements. An analysis of our results reveals the presence of a Cooper minimum in the photoionization of the silyl radical. The adequacy of the two theoretical procedures employed in the present work is discussed.
Interacting Winds in Eclipsing Symbiotic Systems – The Case Study ...
Indian Academy of Sciences (India)
produced by the collision of two stellar winds (Vogel 1991, 1993; Girard & Willson ... Therefore, in the nebular environment an energetic zone .... 1b and 1d). .... By applying Kepler's second law, we obtain the time required to cover the corre-.
Stöhlker, T; Ma, X; Ludziejewski, T; Beyer, H F; Bosch, F; Brinzanescu, O; Dunford, R W; Eichler, J; Hagmann, S; Ichihara, A; Kozhuharov, C; Krämer, A; Liesen, D; Mokler, P H; Stachura, Z; Swiat, P; Warczak, A
2001-02-05
Radiative electron capture, the time-reversed photoionization process occurring in ion-atom collisions, provides presently the only access to photoionization studies for very highly charged ions. By applying the deceleration mode of the ESR storage ring, we studied this process in low-energy collisions of bare uranium ions with low- Z target atoms. This technique allows us to extend the current information about photoionization to much lower energies than those accessible for neutral heavy elements in the direct reaction channel. The results prove that for high- Z systems, higher-order multipole contributions and magnetic corrections persist even at energies close to the threshold.
International Nuclear Information System (INIS)
Hemmers, O.; Lindle, D.W.; Baker, J.; Hudson, A.; Lotrakul, M.; Tran, I.C.; Guillemin, R.; Stolte, W.C.; Wolska, A.; Yu, S.W.; Kanter, E.P.; Kraessig, B.; Southworth, S.H.; Wehlitz, R.; Rolles, D.; Amusia, M.Ya.; Cheng, K.T.; Chernysheva, L.V.; Johnson, W.R.; Manson, S.T.
2003-01-01
The Xe 5s nondipole photoelectron parameter γ is obtained experimentally and theoretically from threshold to ∼200 eV photon energy. Significant nondipole effects are seen even in the threshold region of this valence shell photoionization. In addition, contrary to previous understanding, clear evidence of interchannel coupling among quadrupole photoionization channels is found
Theory of radiatively driven stellar winds. I. A physical interpretation
International Nuclear Information System (INIS)
Abbott, D.C.
1980-01-01
This series of papers extends the line-driven wind theory of Castor, Abbott, and Klein (CAK). The present paper develops a physical interpretation of line-driven flows using analytic methods. Numerical results will follow in two subsequent papers
A vacuum ultraviolet photoionization study on the thermal decomposition of ammonium perchlorate
Góbi, Sándor; Zhao, Long; Xu, Bo; Ablikim, Utuq; Ahmed, Musahid; Kaiser, Ralf I.
2018-01-01
Pyrolysis products of ammonium perchlorate (NH4ClO4) at 483 K were monitored on line and in situ via single photon photoionization reflectron time-of-flight spectrometry (PI-ReTOF-MS) in the photon energy range of 9.00-17.50 eV. The photoionization efficiency curves (PIE) of the subliming product molecules were collected and allowed for detection of three class of products containing chlorine, nitrogen, and oxygen including atoms and free radicals. These results suggest a new insight into possible low-temperature decomposition pathways of NH4ClO4.
Concept, production and validation of a 3D-printed coil frame for the UST2 modular stellarator
International Nuclear Information System (INIS)
Queral, V.
2014-01-01
Highlights: •A construction method for stellarator modular coils is developed and validated. •3D printed truss structure filled and moulded with a material able to solidify. •The structure capability for forces in small stellarators has been estimated. •A light bare truss frame and a covered rigid double hull frame have been tested. -- Abstract: Geometric complexity of stellarators hampers a straightforward production of conceived optimised magnetic configurations. Integration of the engineering design with new fabrication methods may reduce the production cost and accelerate the production process. A fast cycle production of experimental fusion devices also might result in a faster advance in fusion plasma science. Several different stellarators could be used to test configurations for improved turbulent transport or to validate new divertor configurations. In this framework, and based on the results from the previously built UST 1 stellarator, the present work try to study and validate the feasibility of 3D printing methods (additive manufacturing) for small experimental stellarators. The paper summarises the engineering development, fabrication and validation of a coil frame test sector for the UST 2 stellarator. The definition of the Last Closed Flux Surface and winding surface for the test sector is based on an optimised quasi-isodynamic poloidal stellarator, modified for enhanced in-vessel remote handling manipulation and wide space for divertors. A Filled-sparse coil frame concept is developed to still keep low the cost in spite of the present expensive 3D printing materials and printers
International Nuclear Information System (INIS)
Savukov, I. M.; Filin, D. V.
2014-01-01
Many applications are in need of accurate photoionization cross sections, especially in the case of complex atoms. Configuration-interaction relativistic-many-body-perturbation theory (CI-RMBPT) has been successful in predicting atomic energies, matrix elements between discrete states, and other properties, which is quite promising, but it has not been applied to photoionization problems owing to extra complications arising from continuum states. In this paper a method that will allow the conversion of discrete CI-(R)MPBT oscillator strengths (OS) to photoionization cross sections with minimal modifications of the codes is introduced and CI-RMBPT cross sections of Ne, Ar, Kr, and Xe are calculated. A consistent agreement with experiment is found. RMBPT corrections are particularly significant for Ar, Kr, and Xe and improve agreement with experimental results compared to the particle-hole CI method. As a result, the demonstrated conversion method can be applied to CI-RMBPT photoionization calculations for a large number of multivalence atoms and ions
International Nuclear Information System (INIS)
Mandal, P.K.; Seema, A.U.; Das, R.C.; Shah, M.L.; Dev, Vas; Suri, B.M.
2013-01-01
Three-colour three-step photoionization spectroscopy of uranium has been performed in a U–Ne hollow cathode discharge tube by temporally resolving three-colour photoionization optogalvanic (PIOG) signal from the normal optogalvanic (OG) signal using three tunable pulsed dye lasers. U–Ne hollow cathode discharge tube has been used as a source of uranium atomic vapours and photoionization detector. Using this technique, photoionization spectra of uranium have been investigated systematically in the energy region 52,150–52,590 cm −1 , through three different excitation pathways, originating from its ground state, 0 cm −1 ( 5 L o 6 ). By analysing the three-colour photoionization spectra sixty new even-parity autoionization resonances of uranium have been identified and their probable total angular momentum (J) values have been assigned according to the J-momentum selection rule. The J-value of five autoionization resonances, which have been observed either through all three excitation pathways or through two different excitation pathways where J-value of the second excited levels differs by two, has been assigned uniquely. -- Highlights: ► Three-colour photoionization optogalvanic spectroscopy of uranium was performed in a U–Ne hollow cathode discharge tube. ► Hollow cathode discharge tube was used as a source of atomic vapour and laser ionisation detector. ► Uranium photoionization spectra were investigated through three different three-colour photoionization schemes. ► Sixty new even-parity autoionization levels of uranium were identified. ► J-value of five autoionization levels was assigned uniquely
Selective photoionization of gadolinium isotopes with a polarized laser
International Nuclear Information System (INIS)
Le Guyadec, E.
1990-06-01
The aim of this study is the use of gadolinium 157 as burnable poison in nuclear reactors. Spectroscopic isotopic displacements between Gd 156 and Gd 157 are low and the separation method studied is based on differentiated behavior, concerning polarized light, of even and odd gadolinium isotopes coming from their difference of nuclear spin. On this principle is based the simplest photoionization scheme. Selective ionization of odd isotopes is realized from the fundamental state with three resonating photons colinearly polarized. The experimental study confirms the possibility of efficient photoionization. The measured selectivity between Gd 157 and even isotope is over 48 in defined conditions because it can be destroyed by a magnetic field or if photons are not well polarized. Calculations and observations are in good agreement. Odd gadolinium isotope separation is feasible and effects preventing separation are evidenced [fr
Photoionization of Endohedral Atoms: Collective, Reflective and Collateral Emissions
International Nuclear Information System (INIS)
Chakraborty, Himadri S.; McCune, Matthew A.; Hopper, Dale E.; Madjet, Mohamed E.; Manson, Steven T.
2009-01-01
The photoionization properties of a fullerene-confined atom differ dramatically from that of an isolated atom. In the low energy region, where the fullerene plasmons are active, the electrons of the confined atom emerge through a collective channel carrying a significant chunk of plasmon with it. The photoelectron angular distribution of the confined atom however shows far lesser impact of the effect. At higher energies, the interference between two single-electron ionization channels, one directly from the atom and another reflected off the fullerene cage, producuces oscillatory cross sections. But for the outermost atomic level, which transfers some electrons to the cage, oscillations are further modulated by the collateral emission from the part of the atomic charge density transferred to the cage. These various modes of emissions are studied for the photoionization of Ar endohedrally confined in C 60 .
The metastable dynamo model of stellar rotational evolution
International Nuclear Information System (INIS)
Brown, Timothy M.
2014-01-01
This paper introduces a new empirical model for the rotational evolution of Sun-like stars—those with surface convection zones and non-convective interior regions. Previous models do not match the morphology of observed (rotation period)-color diagrams, notably the existence of a relatively long-lived 'C-sequence' of fast rotators first identified by Barnes. This failure motivates the Metastable Dynamo Model (MDM) described here. The MDM posits that stars are born with their magnetic dynamos operating in a mode that couples very weakly to the stellar wind, so their (initially very short) rotation periods at first change little with time. At some point, this mode spontaneously and randomly changes to a strongly coupled mode, the transition occurring with a mass-dependent lifetime that is of the order of 100 Myr. I show that with this assumption, one can obtain good fits to observations of young clusters, particularly for ages of 150-200 Myr. Previous models and the MDM both give qualitative agreement with the morphology of the slower-rotating 'I-sequence' stars, but none of them have been shown to accurately reproduce the stellar-mass-dependent evolution of the I-sequence stars, especially for clusters older than a few hundred million years. I discuss observational experiments that can test aspects of the MDM, and speculate that the physics underlying the MDM may be related to other situations described in the literature, in which stellar dynamos may have a multi-modal character.
The Solar Wind Environment in Time
Pognan, Quentin; Garraffo, Cecilia; Cohen, Ofer; Drake, Jeremy J.
2018-03-01
We use magnetograms of eight solar analogs of ages 30 Myr–3.6 Gyr obtained from Zeeman Doppler Imaging and taken from the literature, together with two solar magnetograms, to drive magnetohydrodynamical wind simulations and construct an evolutionary scenario of the solar wind environment and its angular momentum loss rate. With observed magnetograms of the radial field strength as the only variant in the wind model, we find that a power-law model fitted to the derived angular momentum loss rate against time, t, results in a spin-down relation Ω ∝ t ‑0.51, for angular speed Ω, which is remarkably consistent with the well-established Skumanich law Ω ∝ t ‑0.5. We use the model wind conditions to estimate the magnetospheric standoff distances for an Earth-like test planet situated at 1 au for each of the stellar cases, and to obtain trends of minimum and maximum wind ram pressure and average ram pressure in the solar system through time. The wind ram pressure declines with time as \\overline{{P}ram}}\\propto {t}2/3, amounting to a factor of 50 or so over the present lifetime of the solar system.
Symonds, Joshua M; Gann, Reuben N; Fernández, Facundo M; Orlando, Thomas M
2014-09-01
In this paper, we demonstrate the first use of an atmospheric pressure microplasma-based vacuum ultraviolet (VUV) photoionization source in atmospheric pressure mass spectrometry applications. The device is a robust, easy-to-operate microhollow cathode discharge (MHCD) that enables generation of VUV photons from Ne and Ne/H(2) gas mixtures. Photons were detected by excitation of a microchannel plate detector and by analysis of diagnostic sample ions using a mass spectrometer. Reactive ions, charged particles, and metastables produced in the discharge were blocked from entering the ionization region by means of a lithium fluoride window, and photoionization was performed in a nitrogen-purged environment. By reducing the output pressure of the MHCD, we observed heightened production of higher-energy photons, making the photoionization source more effective. The initial performance of the MHCD VUV source has been evaluated by ionizing model analytes such as acetone, azulene, benzene, dimethylaniline, and glycine, which were introduced in solid or liquid phase. These molecules represent species with both high and low proton affinities, and ionization energies ranging from 7.12 to 9.7 eV.
International Nuclear Information System (INIS)
Shah, M.L.
2017-01-01
Laser-induced fluorescence (LIF) and laser-induced photoionization (LIP) are powerful spectroscopic techniques individually. These techniques have been used extensively for studying the atomic spectra. The potential of these two techniques increases enormously when used simultaneously because of their complimentary nature. Among these two, the resonance ionization spectroscopy is most sensitive, but in some cases the spectra obtained using this photoionization technique can provide the incomplete atomic energy levels information. The complete energy level information can be obtained when both the LIF and LIP techniques are used simultaneously. These techniques have been developed in our laboratory. By employing together both the LIF and LIP techniques for simultaneous detection and utilization of LIF and LIP signals not only helped in developing new methodologies but also helped in getting complete spectral information apart from the measurements of atomic parameters. For the first time, laser-induced fluorescence and laser-induced photoionization techniques are used simultaneously for the spectroscopic investigations of atoms of lanthanides and actinides. The density matrix (DM) formalism is used to validate the experimental results. (author)
Double-continuum wave functions and double-photoionization cross sections of two-electron systems
International Nuclear Information System (INIS)
Tiwary, S.N.
1996-09-01
The present review briefly presents the growing experimental as well as theoretical interests in recent years in the double-continuum wave functions and double-photoionization cross sections of two-electron systems. The validity of existing double-continuum wave functions is analyzed and the importance of electronic correlations in both the initial as well as final states wave functions involved in the transition amplitude for double-photoionization process is demonstrated. At present, we do not have comprehensive and practical double-continuum wave functions which account the full correlation of two-electron in the continuum. Basic difficulties in making accurate theoretical calculations of double ionization by a single high energy photon especially in the vicinity of the threshold, where the correlation plays an important role, are discussed. Illuminating, illustrative and representative examples are presented in order to show the present status and the progress in this field. Future challenges and directions, in high-precision double-photoionization cross sections calculations, have been discussed and suggested. (author). 133 refs, 9 figs
Energy Technology Data Exchange (ETDEWEB)
Neilson, Hilding R.; Lester, John B. [Department of Astronomy and Astrophysics, University of Toronto, 50 St. George Street, Toronto, ON, M5S 3H4 (Canada); Baron, Fabien; Norris, Ryan; Kloppenborg, Brian, E-mail: neilson@astro.utoronto.ca [Center for High Angular Resolution Astronomy, Department of Physics and Astronomy, Georgia State University, P.O. Box 5060, Atlanta, GA 30302-5060 (United States)
2016-10-20
One of the great challenges of understanding stars is measuring their masses. The best methods for measuring stellar masses include binary interaction, asteroseismology, and stellar evolution models, but these methods are not ideal for red giant and supergiant stars. In this work, we propose a novel method for inferring stellar masses of evolved red giant and supergiant stars using interferometric and spectrophotometric observations combined with spherical model stellar atmospheres to measure what we call the stellar mass index, defined as the ratio between the stellar radius and mass. The method is based on the correlation between different measurements of angular diameter, used as a proxy for atmospheric extension, and fundamental stellar parameters. For a given star, spectrophotometry measures the Rosseland angular diameter while interferometric observations generally probe a larger limb-darkened angular diameter. The ratio of these two angular diameters is proportional to the relative extension of the stellar atmosphere, which is strongly correlated to the star’s effective temperature, radius, and mass. We show that these correlations are strong and can lead to precise measurements of stellar masses.
The fundamentals of stellar astrophysics
International Nuclear Information System (INIS)
Collins, G.W. II.
1989-01-01
A broad overview of theoretical stellar astrophysics is presented in a textbook intended for graduate students. Chapters are devoted to fundamental principles, assumptions, theorems, and polytropes; energy sources and sinks; the flow of energy through the star and the construction of stellar models; the theory of stellar evolution; relativistic stellar structure; the structure of distorted stars; stellar pulsation and oscillation. Also discussed are the flow of radiation through the stellar atmosphere, the solution of the radiative-transfer equation, the environment of the radiation field, the construction of a stellar model atmosphere, the formation and shape of spectral lines, LTE breakdown, illuminated and extended stellar atmospheres, and the transfer of polarized radiation. Diagrams, graphs, and sample problems are provided. 164 refs
Separation of uranium isotopes by selective photoionization
International Nuclear Information System (INIS)
Snavely, B.B.; Solarz, R.W.; Tuccio, S.A.
1975-01-01
Recent results of experiments on the laser photoseparation of U isotopes are reported. In the first series of experiments a two-step ionization process using a Xe laser to excite the atoms below the ionization level and then a Kr laser to ionize the atoms was described. Under the geometric conditions of the experiment and power of the Kr laser, enrichments between 2.5 and 3 percent were obtained in runs lasting 2 hrs. Calculations to describe the ion trajectories in the collector system reflected the two-band pattern observed on the Be collector plate. A system to study the photoionization process was assembled in which the U beam is excited to a desired energy level with a CW dye laser and an ultraviolet beam intercepts the excited U beam. An analysis of a photoionization spectrum obtained at a resolution of 8 A indicates that the peak cross section for transitions to autoionization states from the 7 M 7 level is large enough to be used in large-scale U separation systems. An ionization value of 6.15 +- 0.2 eV was deduced for the ionization potential of the U atom. (U.S.)
ON THE LAUNCHING AND STRUCTURE OF RADIATIVELY DRIVEN WINDS IN WOLF–RAYET STARS
Energy Technology Data Exchange (ETDEWEB)
Ro, Stephen; Matzner, Christopher D., E-mail: ro@astro.utoronto.ca [Department of Astronomy and Astrophysics, University of Toronto, 50 St. George Street, Toronto, ON M5S 3H4 (Canada)
2016-04-20
Hydrostatic models of Wolf–Rayet (WR) stars typically contain low-density outer envelopes that inflate the stellar radii by a factor of several and are capped by a denser shell of gas. Inflated envelopes and density inversions are hallmarks of envelopes that become super-Eddington as they cross the iron-group opacity peak, but these features disappear when mass loss is sufficiently rapid. We re-examine the structures of steady, spherically symmetric wind solutions that cross a sonic point at high optical depth, identifying the physical mechanism through which the outflow affects the stellar structure, and provide an improved analytical estimate for the critical mass-loss rate above which extended structures are erased. Weak-flow solutions below this limit resemble hydrostatic stars even in supersonic zones; however, we infer that these fail to successfully launch optically thick winds. WR envelopes will therefore likely correspond to the strong, compact solutions. We also find that wind solutions with negligible gas pressure are stably stratified at and below the sonic point. This implies that convection is not the source of variability in WR stars, as has been suggested; however, acoustic instabilities provide an alternative explanation. Our solutions are limited to high optical depths by our neglect of Doppler enhancements to the opacity, and do not account for acoustic instabilities at high Eddington factors; yet, they do provide useful insights into WR stellar structures.
Internal energy selection in vacuum ultraviolet photoionization of ethanol and ethanol dimers
Bodi, Andras
2013-10-01
Internal energy selected ethanol monomer and ethanol dimer ions were prepared by threshold photoionization of a supersonic molecular beam seeded with ethanol. The dissociative photoionization processes of the monomer, the lowest-energy CH3-loss channel of the dimer, and the fragmentation of larger clusters were found to be disjunct from the ionization onset to about 12 eV, which made it possible to determine the 0 K appearance energy of C-C bond breaking in the H-donor unit of the ethanol dimer cation as 9.719 ± 0.004 eV. This reaction energy is used together with ab initio calculations in a thermochemical cycle to determine the binding energy change from the neutral ethanol dimer to a protonated ethanol-formaldehyde adduct. The cycle also shows general agreement between experiment, theory, and previously published enthalpies of formation. The role of the initial ionization site, or rather the initial photoion state, is also discussed based on the dimer breakdown diagram and excited state calculations. There is no evidence for isolated state behavior, and the ethanol dimer dissociative photoionization processes appear to be governed by statistical theory and the ground electronic state of the ion. In the monomer breakdown diagram, the smoothly changing branching ratio between H and CH3 loss is at odds with rate theory predictions, and shows that none of the currently employed few-parameter rate models, appropriate for experimental rate curve fitting, yields a correct description for this process in the experimental energy range.
Winfough, Matthew; Meloni, Giovanni
2017-12-01
Absolute photoionization cross sections for 2 potential propargylic fuels (propargylamine and dipropargyl ether) along with the partial ionization cross sections for their dissociative fragments are measured and presented for the first time via synchrotron photoionization mass spectrometry. The experimental setup consists of a multiplexed orthogonal time-of-flight mass spectrometer and is located at the Advanced Light Source facility of the Lawrence Berkeley National Laboratory in Berkeley, California. Data for a third propargylic compound (propargyl alcohol) were taken; however, because of its low signal, due to its weakly bound cation, only the dissociative ionization fragment from the H-loss channel is observed and presented. Suggested pathways leading to formation of dissociative photoionization fragments along with CBS-QB3 calculated adiabatic ionization energies and appearance energies for the dissociative fragments are also presented. Copyright © 2017 John Wiley & Sons, Ltd.
Photoelectron wave function in photoionization: plane wave or Coulomb wave?
Gozem, Samer; Gunina, Anastasia O; Ichino, Takatoshi; Osborn, David L; Stanton, John F; Krylov, Anna I
2015-11-19
The calculation of absolute total cross sections requires accurate wave functions of the photoelectron and of the initial and final states of the system. The essential information contained in the latter two can be condensed into a Dyson orbital. We employ correlated Dyson orbitals and test approximate treatments of the photoelectron wave function, that is, plane and Coulomb waves, by comparing computed and experimental photoionization and photodetachment spectra. We find that in anions, a plane wave treatment of the photoelectron provides a good description of photodetachment spectra. For photoionization of neutral atoms or molecules with one heavy atom, the photoelectron wave function must be treated as a Coulomb wave to account for the interaction of the photoelectron with the +1 charge of the ionized core. For larger molecules, the best agreement with experiment is often achieved by using a Coulomb wave with a partial (effective) charge smaller than unity. This likely derives from the fact that the effective charge at the centroid of the Dyson orbital, which serves as the origin of the spherical wave expansion, is smaller than the total charge of a polyatomic cation. The results suggest that accurate molecular photoionization cross sections can be computed with a modified central potential model that accounts for the nonspherical charge distribution of the core by adjusting the charge in the center of the expansion.
International Nuclear Information System (INIS)
Lin, C.Y.; Ho, Y.K.
2010-01-01
The screening effects due to the exponential-cosine-screened Coulomb and screened Coulomb (Yukawa) potentials on photoionization processes are explored within the framework of complex coordinate rotation method. The energy levels of H and He + in both screened potentials shifted with various Debye screening lengths are presented. The photoionization cross sections illustrate the considerable screening effects on photoionization processes in low energy region. The shape resonances can be found near ionization thresholds for certain of Debye screening lengths. The relations between the appearance of resonances and the existence of quasi-bound states under shielding conditions are discussed. (authors)
Energy Technology Data Exchange (ETDEWEB)
Réville, Victor; Brun, Allan Sacha; Strugarek, Antoine; Pinto, Rui F. [Laboratoire AIM, DSM/IRFU/SAp, CEA Saclay, F-91191 Gif-sur-Yvette Cedex (France); Matt, Sean P., E-mail: victor.reville@cea.fr, E-mail: sacha.brun@cea.fr, E-mail: s.matt@exeter.ac.uk, E-mail: strugarek@astro.umontreal.ca, E-mail: rui.pinto@obspm.fr [Department of Physics and Astronomy, University of Exeter, Stocker Road, Exeter EX4 4SB (United Kingdom)
2015-01-10
Stellar wind is thought to be the main process responsible for the spin down of main-sequence stars. The extraction of angular momentum by a magnetized wind has been studied for decades, leading to several formulations for the resulting torque. However, previous studies generally consider simple dipole or split monopole stellar magnetic topologies. Here we consider, in addition to a dipolar stellar magnetic field, both quadrupolar and octupolar configurations, while also varying the rotation rate and the magnetic field strength. Sixty simulations made with a 2.5D cylindrical and axisymmetric set-up, and computed with the PLUTO code, were used to find torque formulations for each topology. We further succeed to give a unique law that fits the data for every topology by formulating the torque in terms of the amount of open magnetic flux in the wind. We also show that our formulation can be applied to even more realistic magnetic topologies, with examples of the Sun in its minimum and maximum phases as observed at the Wilcox Solar Observatory, and of a young K-star (TYC-0486-4943-1) whose topology has been obtained by Zeeman-Doppler Imaging.
Photoionization cross-section of thallium 7 2D5/2 state at 1.06 μm radiation
International Nuclear Information System (INIS)
Ko, Kwang Hoon; Jeong, Do Young; Lim, Gwon; Kim, Jae Woo; Kim, Taek Soo; Rho, Si Pyo; Kim, Cheol Jung
2003-01-01
Thallium has two naturally occurring isotopes of T1-203 and T1-205, which have abundances of 30% and 70%, respectively. Development of the isotope separation technique of T1-203 has been attractive due to its industrial demand. T1-203 is raw material for production of T1-201 radioisotopes by proton bombardment in a cyclotron. The final product of 2 01 'T1C1 radiopharmaceuticals is widely used to diagnose heart disease. Electric field ionization has been proposed for isotope selective ionization of thallium atoms but it is not adequate to produce massive thallium ions. We report the result of infra-red (IR) photoionization experiment of thallium atoms. The measures photoionization cross-section of 7 2 D 5/2 state of atoms was at 1.06 μm radiation, which means that ionization efficiency higher than 80% can be achieved with a pulsed Nd:YAG laser of pulse energy density of about. For the accurate determination of the photoionization cross-section, calibration of the linearity of a energy meter should be performed. Density matrix equations were employed for the simulation of the photoionization process and its results were used to determine the photoionization cross-section.
SDP_golofs01_3: Stellar Disk Evolution
Olofsson, G.
2010-03-01
n a collaboration between the HSC, P. Harvey (Mission Scientist) and the three instrument consortia we propose to apply the full power of Herschel to investigate the properties of circum-stellar disks. The versatility of Herschel allows us to address several key questions: How do the disks evolve with time? Planets clearly form out of circum-stellar disks and there is growing evidence that the time scale is short, 1 - 10 Myr, for the main accretion phase. During this time period, the stellar radiation and stellar winds clean the disks from most of their dust and gas, eventually making them transparent. However, collisions and evaporation from comet- like bodies will continue to produce dust and gas. This activity declines with time, and we will pursue this scenario by observing a sample of IR excess stars of known age, ranging from a few million years to the age of the sun. Are there analogues to our Kuiper belt around nearby stars? The Kuiper belt is a dust belt surrounding the Sun, located outside the orbit of Neptune, which has a key role in stabilizing orbits of the KE-objects and this dynamical aspect makes it particularly interesting to search for stars that may host KE-belt analogues. Herschel offers a unique sensitivity beyond 100 m and we propose an extensive survey of nearby stars seeking cold dust emission. What will a closer IR look at the "Fabulous Four" (and some other resolved disks) reveal? Several nearby MS stars with IR excesses have circumstellar dust structures that can be resolved by Herschel. Imaging these structures in the six PACS+SPIRE bands will enable us to explore the dust properties, notably the size distribution and albedo.. What is the composition of young disks? We propose a detailed spectroscopic investigation of four bright disks, including a full spectral scan with PACS, an FTS scan at full resolution and HIFI observations of selected frequencies. The aim is to constrain the properties of both the dust and gas components.
A non-invasive online photoionization spectrometer for FLASH2.
Braune, Markus; Brenner, Günter; Dziarzhytski, Siarhei; Juranić, Pavle; Sorokin, Andrey; Tiedtke, Kai
2016-01-01
The stochastic nature of the self-amplified spontaneous emission (SASE) process of free-electron lasers (FELs) effects pulse-to-pulse fluctuations of the radiation properties, such as the photon energy, which are determinative for processes of photon-matter interactions. Hence, SASE FEL sources pose a great challenge for scientific investigations, since experimenters need to obtain precise real-time feedback of these properties for each individual photon bunch for interpretation of the experimental data. Furthermore, any device developed to deliver the according information should not significantly interfere with or degrade the FEL beam. Regarding the spectral properties, a device for online monitoring of FEL wavelengths has been developed for FLASH2, which is based on photoionization of gaseous targets and the measurements of the corresponding electron and ion time-of-flight spectra. This paper presents experimental studies and cross-calibration measurements demonstrating the viability of this online photoionization spectrometer.
Dissociative Photoionization of 1-Halogenated Silacyclohexanes: Silicon Traps the Halogen.
Bodi, Andras; Sigurdardottir, Katrin Lilja; Kvaran, Ágúst; Bjornsson, Ragnar; Arnason, Ingvar
2016-11-23
The threshold photoelectron spectra and threshold photoionization mass spectra of 1-halogenated-1-silacyclohexanes, for the halogens X = F, Cl, Br, and I, have been obtained using synchrotron vacuum ultraviolet radiation and photoelectron photoion coincidence spectroscopy. As confirmed by a similar ionization onset and density functional theory molecular orbitals, the ionization to the ground state is dominated by electron removal from the silacyclohexane ring for X = F, Cl, and Br, and from the halogen lone pair for X = I. The breakdown diagrams show that the dissociative photoionization mechanism is also different for X = I. Whereas the parent ions decay by ethylene loss for X = F to Br in the low-energy regime, the iodine atom is lost for X = I. The first step is followed by a sequential ethylene loss at higher internal energies in each of the compounds. It is argued that the tendency of silicon to lower bond angles stabilizes the complex cation in which C 2 H 4 is η 2 -coordinated to it, and which precedes ethylene loss. Together with the relatively strong silicon-halogen bonds and the increased inductive effect of the silacyclohexane ring in stabilizing the cation, this explains the main differences observed in the fragmentation of the halogenated silacyclohexane and halogenated cyclohexane ions. The breakdown diagrams have been modeled taking into account slow dissociations at threshold and the resulting kinetic shift. The 0 K appearance energies have been obtained to within 0.08 eV for the ethylene loss for X = F to Br (10.56, 10.51, and 10.51 eV, respectively), the iodine atom loss for X = I (10.11 eV), the sequential ethylene loss for X = F to I (12.29, 12.01, 11.94, and 11.86 eV, respectively), and the minor channels of H loss for X = F (10.56 eV) and propylene loss in X = Cl (also at 10.56 eV). The appearance energies for the major channels likely correspond to the dissociative photoionization reaction energy.
Nahar, S. N.
2003-01-01
Most astrophysical plasmas entail a balance between ionization and recombination. We present new results from a unified method for self-consistent and ab initio calculations for the inverse processes of photoionization and (e + ion) recombination. The treatment for (e + ion) recombination subsumes the non-resonant radiative recombination and the resonant dielectronic recombination processes in a unified scheme (S.N. Nahar and A.K. Pradhan, Phys. Rev. A 49, 1816 (1994);H.L. Zhang, S.N. Nahar, and A.K. Pradhan, J.Phys.B, 32,1459 (1999)). Calculations are carried out using the R-matrix method in the close coupling approximation using an identical wavefunction expansion for both processes to ensure self-consistency. The results for photoionization and recombination cross sections may also be compared with state-of-the-art experiments on synchrotron radiation sources for photoionization, and on heavy ion storage rings for recombination. The new experiments display heretofore unprecedented detail in terms of resonances and background cross sections and thereby calibrate the theoretical data precisely. We find a level of agreement between theory and experiment at about 10% for not only the ground state but also the metastable states. The recent experiments therefore verify the estimated accuracy of the vast amount of photoionization data computed under the OP, IP and related works. features. Present work also reports photoionization cross sections including relativistic effects in the Breit-Pauli R-matrix (BPRM) approximation. Detailed features in the calculated cross sections exhibit the missing resonances due to fine structure. Self-consistent datasets for photoionization and recombination have so far been computed for approximately 45 atoms and ions. These are being reported in a continuing series of publications in Astrophysical J. Supplements (e.g. references below). These data will also be available from the electronic database TIPTOPBASE (http://heasarc.gsfc.nasa.gov)
Alpha-particle confinement and helium ash accumulation in stellarator reactors
International Nuclear Information System (INIS)
Ho, D.D.-M.; Kulsrud, R.M.
1986-01-01
The effect of local magnetic wells produced by the external helical windings of a stellarator reactor on α-particle confinement is investigated by using the Fokker-Planck equation. It is found that α-particles can deposit most of their energy into the background plasma before they scatter into the trapped region in velocity space and are lost. An estimate is made on the steady-state, low energy (thermal) α-particle concentration. The result shows that this concentration will be less than a few per cent of the background plasma density. (author)
Absolute photoionization cross sections of two cyclic ketones: cyclopentanone and cyclohexanone.
Price, Chelsea; Fathi, Yasmin; Meloni, Giovanni
2017-05-01
Absolute photoionization cross sections for cyclopentanone and cyclohexanone, as well as partial ionization cross sections for the dissociative ionized fragments, are presented in this investigation. Experiments are performed via a multiplexed photoionization mass spectrometer utilizing vacuum ultraviolet (VUV) synchrotron radiation supplied by the Advanced Light Source of Lawrence Berkeley National Laboratory. These results allow the quantification of these species that is relevant to investigate the kinetics and combustion reactions of potential biofuels. The CBS-QB3 calculated values for the adiabatic ionization energies agree well with the experimental values, and the identification of possible dissociative fragments is discussed for both systems. Copyright © 2017 John Wiley & Sons, Ltd. Copyright © 2017 John Wiley & Sons, Ltd.
Spatially resolved photoionization of ultracold atoms on an atom chip
International Nuclear Information System (INIS)
Kraft, S.; Guenther, A.; Fortagh, J.; Zimmermann, C.
2007-01-01
We report on photoionization of ultracold magnetically trapped Rb atoms on an atom chip. The atoms are trapped at 5 μK in a strongly anisotropic trap. Through a hole in the chip with a diameter of 150 μm, two laser beams are focused onto a fraction of the atomic cloud. A first laser beam with a wavelength of 778 nm excites the atoms via a two-photon transition to the 5D level. With a fiber laser at 1080 nm the excited atoms are photoionized. Ionization leads to depletion of the atomic density distribution observed by absorption imaging. The resonant ionization spectrum is reported. The setup used in this experiment is suitable not only to investigate mixtures of Bose-Einstein condensates and ions but also for single-atom detection on an atom chip
International Nuclear Information System (INIS)
Kemeny, P.C.
1974-01-01
Subshell photoionization cross-sections of both core and valence electrons in solid samples of sodium fluoride and sodium chloride were measured at a photon energy of 1487 eV (Al Kα). Relative to the sodium 1s level, values are reported for the subshell photoionization cross-sections of the sodium 2s, 2p, chlorine 2s, 2p, 3s, 3p and fluorine 1s, 2s and 2p levels. Subshell photoionization cross-sections of outer levels in the noble gases neon through xenon were also measured, at photon energies of 21.22, 40.81 and 48.37 eV. Values are reported for the photoionization cross-sections of the neon 2p, krypton 4p, xenon 5p and xenon 5s levels, relative to that of the argon 3p level. Whereever possible, comparison was made between the present relative subshell photoionization cross-section values and those reported by other workers. (author)
Continuum emission from classical nova winds
International Nuclear Information System (INIS)
Harkness, R.P.
1983-01-01
The emergent continuum of a slow classical nova during outburst is considered in the quasi-steady optically thick, transonic wind model. Models are presented for various steady mass loss rates and are related to the evolution of slow novae during decline and early post-maximum. The continuum emission is found to depart radically from a blackbody spectrum and to exhibit features common to highly extended stellar atmospheres. (author)
Infrared laser ablation atmospheric pressure photoionization mass spectrometry.
Vaikkinen, Anu; Shrestha, Bindesh; Kauppila, Tiina J; Vertes, Akos; Kostiainen, Risto
2012-02-07
In this paper we introduce laser ablation atmospheric pressure photoionization (LAAPPI), a novel atmospheric pressure ion source for mass spectrometry. In LAAPPI the analytes are ablated from water-rich solid samples or from aqueous solutions with an infrared (IR) laser running at 2.94 μm wavelength. Approximately 12 mm above the sample surface, the ablation plume is intercepted with an orthogonal hot solvent (e.g., toluene or anisole) jet, which is generated by a heated nebulizer microchip and directed toward the mass spectrometer inlet. The ablated analytes are desolvated and ionized in the gas-phase by atmospheric pressure photoionization using a 10 eV vacuum ultraviolet krypton discharge lamp. The effect of operational parameters and spray solvent on the performance of LAAPPI is studied. LAAPPI offers ~300 μm lateral resolution comparable to, e.g., matrix-assisted laser desorption ionization. In addition to polar compounds, LAAPPI efficiently ionizes neutral and nonpolar compounds. The bioanalytical application of the method is demonstrated by the direct LAAPPI analysis of rat brain tissue sections and sour orange (Citrus aurantium) leaves. © 2012 American Chemical Society
International Nuclear Information System (INIS)
Natalense, Alexandra P. P.; Brescansin, Luiz M.; Lucchese, Robert R.
2003-01-01
We have computed cross sections and asymmetry parameters for the C 1s photoionization of CX 4 (X=H, F, Cl) using the Schwinger variational method with Pade corrections. We present a comparative study that shows the influence of the identity of the X atom on the computed cross sections. Predicted cross sections are in good agreement with available photoionization and photoabsorption experimental data. We conclude that the presence of heavy outer atoms produces resonance structures in the photoionization cross sections and in the asymmetry parameters. We find a single nonvalence resonant state in the photoionization of CF 4 and multiple resonances in CCl 4 that have significant d-orbital character in the vicinity of the Cl atoms
Stener, M; Bolognesi, P; Coreno, M; O'Keeffe, P; Feyer, V; Fronzoni, G; Decleva, P; Avaldi, L; Kivimäki, A
2011-05-07
Photoabsorption and S 2p photoionization of the SF(6) molecule have been studied experimentally and theoretically in the excitation energy range up to 100 eV above the S 2p ionization potentials. In addition to the well-known 2t(2g) and 4e(g) shape resonances, the spin-orbit-resolved S 2p photoionization cross sections display two weak resonances between 200 and 210 eV, a wide resonance around 217 eV, a Fano-type resonance around 240 eV, and a second wide resonance around 260 eV. Calculations based on time-dependent density functional theory allow us to assign the 217-eV and 260-eV features to the shape resonances in S 2p photoionization. The Fano resonance is caused by the interference between the direct S 2p photoionization channel and the resonant channel that results from the participator decay of the S 2s(-1)6t(1u) excited state. The weak resonances below 210-eV photon energy, not predicted by theory, are tentatively suggested to originate from the coupling between S 2p shake-up photoionization and S 2p single-hole photoionization. The experimental and calculated angular anisotropy parameters for S 2p photoionization are in good agreement.
Gans, Bérenger; Garcia, Gustavo A; Boyé-Péronne, Séverine; Loison, Jean-Christophe; Douin, Stéphane; Gaie-Levrel, François; Gauyacq, Dolores
2011-06-02
The absolute photoionization cross section of C(2)H(5) has been measured at 10.54 eV using vacuum ultraviolet (VUV) laser photoionization. The C(2)H(5) radical was produced in situ using the rapid C(2)H(6) + F → C(2)H(5) + HF reaction. Its absolute photoionization cross section has been determined in two different ways: first using the C(2)H(5) + NO(2) → C(2)H(5)O + NO reaction in a fast flow reactor, and the known absolute photoionization cross section of NO. In a second experiment, it has been measured relative to the known absolute photoionization cross section of CH(3) as a reference by using the CH(4) + F → CH(3) + HF and C(2)H(6) + F → C(2)H(5) + HF reactions successively. Both methods gave similar results, the second one being more precise and yielding the value: σ(C(2)H(5))(ion) = (5.6 ± 1.4) Mb at 10.54 eV. This value is used to calibrate on an absolute scale the photoionization curve of C(2)H(5) produced in a pyrolytic source from the C(2)H(5)NO(2) precursor, and ionized by the VUV beam of the DESIRS beamline at SOLEIL synchrotron facility. In this latter experiment, a recently developed ion imaging technique is used to discriminate the direct photoionization process from dissociative ionization contributions to the C(2)H(5)(+) signal. The imaging technique applied on the photoelectron signal also allows a slow photoelectron spectrum with a 40 meV resolution to be extracted, indicating that photoionization around the adiabatic ionization threshold involves a complex vibrational overlap between the neutral and cationic ground states, as was previously observed in the literature. Comparison with earlier photoionization studies, in particular with the photoionization yield recorded by Ruscic et al. is also discussed. © 2011 American Chemical Society
Compact stellarators as reactors
International Nuclear Information System (INIS)
Lyon, J.F.; Valanju, P.; Zarnstorff, M.C.; Hirshman, S.; Spong, D.A.; Strickler, D.; Williamson, D.E.; Ware, A.
2001-01-01
Two types of compact stellarators are examined as reactors: two- and three-field-period (M=2 and 3) quasi-axisymmetric devices with volume-average =4-5% and M=2 and 3 quasi-poloidal devices with =10-15%. These low-aspect-ratio stellarator-tokamak hybrids differ from conventional stellarators in their use of the plasma-generated bootstrap current to supplement the poloidal field from external coils. Using the ARIES-AT model with B max =12T on the coils gives Compact Stellarator reactors with R=7.3-8.2m, a factor of 2-3 smaller R than other stellarator reactors for the same assumptions, and neutron wall loadings up to 3.7MWm -2 . (author)
Saber, Ismail; Bartnik, Andrzej; Skrzeczanowski, Wojciech; Wachulak, Przemysław; Jarocki, Roman; Fiedorowicz, Henryk
2017-03-01
Experimental measurements and numerical modeling of emission spectra in photoionized plasma in the ultraviolet and visible light (UV/Vis) range for noble gases have been investigated. The photoionized plasmas were created using laser-produced plasma (LPP) extreme ultraviolet (EUV) source. The source was based on a gas puff target; irradiated with 10ns/10J/10Hz Nd:YAG laser. The EUV radiation pulses were collected and focused using grazing incidence multifoil EUV collector. The laser pulses were focused on a gas stream, injected into a vacuum chamber synchronously with the EUV pulses. Irradiation of gases resulted in a formation of low temperature photoionized plasmas emitting radiation in the UV/Vis spectral range. Atomic photoionized plasmas produced this way consisted of atomic and ionic with various ionization states. The most dominated observed spectral lines originated from radiative transitions in singly charged ions. To assist in a theoretical interpretation of the measured spectra, an atomic code based on Cowan's programs and a collisional-radiative PrismSPECT code have been used to calculate the theoretical spectra. A comparison of the calculated spectral lines with experimentally obtained results is presented. Electron temperature in plasma is estimated using the Boltzmann plot method, by an assumption that a local thermodynamic equilibrium (LTE) condition in the plasma is validated in the first few ionization states. A brief discussion for the measured and computed spectra is given.
Photoionization of the hydrogen atom in strong magnetic fields
Potekhin, Aleksandr IU.; Pavlov, George G.
1993-01-01
The photoionization of the hydrogen atom in magnetic fields B about 10 exp 11 - 10 exp 13 G typical of the surface layers of neutron stars is investigated analytically and numerically. We consider the photoionization from various tightly bound and hydrogen-like states of the atom for photons with arbitrary polarizations and wave-vector directions. It is shown that the length form of the interaction matrix elements is more appropriate in the adiabatic approximation than the velocity form, at least in the most important frequency range omega much less than omega(B), where omega(B) is the electron cyclotron frequency. Use of the length form yields nonzero cross sections for photon polarizations perpendicular to the magnetic field at omega less than omega(B); these cross sections are the ones that most strongly affect the properties of the radiation escaping from an optically thick medium, e.g., from the atmosphere of a neutron star. The results of the numerical calculations are fitted by simple analytical formulas.
International Nuclear Information System (INIS)
Schrijver, C.J.
1986-01-01
The stellar emission in the chromospheric Ca II H+K lines is compared with the coronal soft X-ray emission, measuring the effects of non-radiative heating in the outer atmosphere at temperatures differing two orders of magnitude. The comparison of stellar flux densities in Ca II H+K and X-rays is extended to fluxes from the transition-region and the high-temperature chromosphere. The stellar magnetic field is probably generated in the differentially rotating convective envelope. The relation between rotation rate and the stellar level of activity measured in chromospheric, transition-region, and coronal radiative diagnostics is discovered. X-ray observations of the binary λ Andromedae are discussed. The departure of M-type dwarfs from the main relations, and the implications for the structure of the chromospheres of these stars are discussed. Variations of the average surface flux densities of the Sun during the 11-year activity cycle agree with flux-flux relations derived for other cool stars, suggesting that the interpretation of the stellar relations may be furthered by studying the solar analogue in more detail. (Auth.)
Structure and Dynamics of the Accretion Process and Wind in TW Hya
Dupree, A. K.; Brickhouse, N. S.; Cranmer, S. R.; Berlind, P.; Strader, Jay; Smith, Graeme H.
2014-07-01
Time-domain spectroscopy of the classical accreting T Tauri star, TW Hya, covering a decade and spanning the far UV to the near-infrared spectral regions can identify the radiation sources, the atmospheric structure produced by accretion, and properties of the stellar wind. On timescales from days to years, substantial changes occur in emission line profiles and line strengths. Our extensive time-domain spectroscopy suggests that the broad near-IR, optical, and far-uv emission lines, centered on the star, originate in a turbulent post-shock region and can undergo scattering by the overlying stellar wind as well as some absorption from infalling material. Stable absorption features appear in Hα, apparently caused by an accreting column silhouetted in the stellar wind. Inflow of material onto the star is revealed by the near-IR He I 10830 Å line, and its free-fall velocity correlates inversely with the strength of the post-shock emission, consistent with a dipole accretion model. However, the predictions of hydrogen line profiles based on accretion stream models are not well-matched by these observations. Evidence of an accelerating warm to hot stellar wind is shown by the near-IR He I line, and emission profiles of C II, C III, C IV, N V, and O VI. The outflow of material changes substantially in both speed and opacity in the yearly sampling of the near-IR He I line over a decade. Terminal outflow velocities that range from 200 km s-1 to almost 400 km s-1 in He I appear to be directly related to the amount of post-shock emission, giving evidence for an accretion-driven stellar wind. Calculations of the emission from realistic post-shock regions are needed. Data presented herein were obtained at the W. M. Keck Observatory, which is operated as a scientific partnership among the California Institute of Technology, the University of California, and the National Aeronautics and Space Administration. The Observatory was made possible by the generous financial support
A photoionization model for the optical line emission from cooling flows
Donahue, Megan; Voit, G. M.
1991-01-01
The detailed predictions of a photoionization model previously outlined in Voit and Donahue (1990) to explain the optical line emission associated with cooling flows in X-ray emitting clusters of galaxies are presented. In this model, EUV/soft X-ray radiation from condensing gas photoionizes clouds that have already cooled. The energetics and specific consequences of such a model, as compared to other models put forth in the literature is discussed. Also discussed are the consequences of magnetic fields and cloud-cloud shielding. The results illustrate how varying the individual column densities of the ionized clouds can reproduce the range of line ratios observed and strongly suggest that the emission-line nebulae are self-irradiated condensing regions at the centers of cooling flows.
International Nuclear Information System (INIS)
Cool, Terrill A.; Nakajima, Koichi; Mostefaoui, Toufik A.; Qi, Fei; McIlroy, Andrew; Westmoreland, Phillip R.; Law, Matthew E.; Poisson, Lionel; Peterka, Darcy S.; Ahmed, Musahid
2003-01-01
We report the first use of synchrotron radiation, continuously tunable from 8 to 15 eV, for flame-sampling photoionization mass spectrometry (PIMS). Synchrotron radiation offers important advantages over the use of pulsed vacuum ultraviolet lasers for PIMS; these include superior signal-to-noise, soft ionization, and access to photon energies outside the limited tuning ranges of current VUV laser sources. Near-threshold photoionization efficiency measurements were used to determine the absolute concentrations of the allene and propyne isomers of C 3 H 4 in low-pressure laminar ethylene-oxygen and benzene-oxygen flames. Similar measurements of the isomeric composition of C 2 H 4 O species in a fuel-rich ethylene-oxygen flame revealed the presence of substantial concentrations of ethenol (vinyl alcohol) and acetaldehyde. Ethenol has not been previously detected in hydrocarbon flames. Absolute photoionization cross sections were measured for ethylene, allene, propyne, and acetaldehyde, using propene as a calibration standard. PIE curves are presented for several additional reaction intermediates prominent in hydrocarbon flames
Multiple photoionization from 3p excitation of Kr and 4p excitation of Xe
International Nuclear Information System (INIS)
Hayaishi, T.
1986-01-01
The photoionization cross sections for multiply charged ions produced by 3p excitation of Kr and 4p excitation of Xe have been obtained by means of a time-of-flight mass spectrometer and synchrotron radiation. It is found that the main formation of doubly to quadruply charged ions in both Kr and Xe is caused from the each initial p-hole state through a Coster-Kronig transition followed by Auger of double Auger processes. The formation of singly charged ions in these excitation energy regions is caused by direct photoionization from outermost shell electrons in both Kr and Xe. Triply charged ions are prominently produced among the multiply charged ions. The quadruple photoionization cross sections show clearly the structures due to the Rydberg series, 3p -1 nl of Kr and 4p -1 nl of Xe. Their main structures were assigned to the 3p -1 nd series in Kr and the 4p -1 nd series in Xe. (orig.)
Concept, production and validation of a 3D-printed coil frame for the UST{sub 2} modular stellarator
Energy Technology Data Exchange (ETDEWEB)
Queral, V., E-mail: vicentemanuel.queral@ciemat.es
2014-10-15
Highlights: •A construction method for stellarator modular coils is developed and validated. •3D printed truss structure filled and moulded with a material able to solidify. •The structure capability for forces in small stellarators has been estimated. •A light bare truss frame and a covered rigid double hull frame have been tested. -- Abstract: Geometric complexity of stellarators hampers a straightforward production of conceived optimised magnetic configurations. Integration of the engineering design with new fabrication methods may reduce the production cost and accelerate the production process. A fast cycle production of experimental fusion devices also might result in a faster advance in fusion plasma science. Several different stellarators could be used to test configurations for improved turbulent transport or to validate new divertor configurations. In this framework, and based on the results from the previously built UST{sub 1} stellarator, the present work try to study and validate the feasibility of 3D printing methods (additive manufacturing) for small experimental stellarators. The paper summarises the engineering development, fabrication and validation of a coil frame test sector for the UST{sub 2} stellarator. The definition of the Last Closed Flux Surface and winding surface for the test sector is based on an optimised quasi-isodynamic poloidal stellarator, modified for enhanced in-vessel remote handling manipulation and wide space for divertors. A Filled-sparse coil frame concept is developed to still keep low the cost in spite of the present expensive 3D printing materials and printers.
sunstardb: A Database for the Study of Stellar Magnetism and the Solar-stellar Connection
Egeland, Ricky
2018-05-01
The “solar-stellar connection” began as a relatively small field of research focused on understanding the processes that generate magnetic fields in stars and sometimes lead to a cyclic pattern of long-term variability in activity, as demonstrated by our Sun. This area of study has recently become more broadly pertinent to questions of exoplanet habitability and exo-space weather, as well as stellar evolution. In contrast to other areas of stellar research, individual stars in the solar-stellar connection often have a distinct identity and character in the literature, due primarily to the rarity of the decades-long time-series that are necessary for studying stellar activity cycles. Furthermore, the underlying stellar dynamo is not well understood theoretically, and is thought to be sensitive to several stellar properties, e.g., luminosity, differential rotation, and the depth of the convection zone, which in turn are often parameterized by other more readily available properties. Relevant observations are scattered throughout the literature and existing stellar databases, and consolidating information for new studies is a tedious and laborious exercise. To accelerate research in this area I developed sunstardb, a relational database of stellar properties and magnetic activity proxy time-series keyed by individual named stars. The organization of the data eliminates the need for the problematic catalog cross-matching operations inherent when building an analysis data set from heterogeneous sources. In this article I describe the principles behind sunstardb, the data structures and programming interfaces, as well as use cases from solar-stellar connection research.
2002-01-01
[TOP LEFT AND RIGHT] The Hubble Space Telescope's Wide Field and Planetary Camera 2 has captured images of the birth of two planetary nebulae as they emerge from wrappings of gas and dust, like butterflies breaking out of their cocoons. These images highlight a fleeting phase in the stellar burnout process, occurring just before dying stars are transformed into planetary nebulae. The left-hand image is the Cotton Candy nebula, IRAS 17150-3224; the right-hand image, the Silkworm nebula, IRAS 17441-2411. Called proto-planetary nebulae, these dying stars have been caught in a transition phase between a red giant and a planetary nebula. This phase is only about 1,000 years long, very short in comparison to the 1 billion-year lifetime of a star. These images provide the earliest snapshots of the transition process. Studying images of proto-planetary nebulae is important to understanding the process of star death. A star begins to die when it has exhausted its thermonuclear fuel - hydrogen and helium. The star then becomes bright and cool (red giant phase) and swells to several tens of times its normal size. It begins puffing thin shells of gas off into space. These shells become the star's cocoon. In the Hubble images, the shells are the concentric rings seen around each nebula. But the images also reveal the nebulae breaking out from those shells. The butterfly-like wings of gas and dust are a common shape of planetary nebulae. Such butterfly shapes are created by the 'interacting winds' process, in which a more recent 'fast wind' - material propelled by radiation from the hot central star - punches a hole in the cocoon, allowing the nebula to emerge. (This 'interacting wind' theory was first proposed by Dr. Sun Kwok to explain the origin of planetary nebulae, and has been subsequently proven successful in explaining their shapes.) The nebulae are being illuminated by light from the invisible central star, which is then reflected toward us. We are viewing the nebulae
New photoionization lasers pumped by laser-induced plasma radiation
International Nuclear Information System (INIS)
Hube, M.; Dieckmann, M.; Beigang, R.; Welling, H.; Wellegehausen, B.
1988-01-01
Innershell photoionization of atomic gases and vapors by soft x rays from a laser-produced plasma is a potential method for making lasers at short wavelengths. Normally, in such experiments only a single plasma spot or plasma line is created for the excitation. This gives high excitation rates but only a short excitation length. At high excitation rates detrimental influences, such as amplified spontaneous emission, optical saturation, or quenching processes, may decrease or even destroy a possible inversion. Therefore, it seems to be more favorable to use a number of separated plasma spots with smaller excitation rates and larger excitation lengths. As a test, a three-plasma spot device was constructed and used in the well-known Cd-photoionization laser at 442 nm. With a 600-mJ Nd:YAH laser (pulse length, 8 ns) for plasma production, output energies up to 300 μJ have been measured, which is more than a doubling of so far obtained data. On innershell excitation, levels may be populated that allow direct lasers as in the case of Cd or that are metastable and cannot be directly coupled to lower levels. In this case modifications in the excitation process are necessary. Such modifications may be an optical pump process in the atom prior to the innershell photoionization or an optical pump process (population transfer process) after the innershell ionization, leading to Raman or anti-Stokes Raman-type laser emissions. With these techniques and the developed multiplasma spot excitation device a variety of new laser emissions in K and Cs ions have been achieved which are indicated in the level schemes
Sun, W. Q.; Shu, J. N.; Zhang, P.; Li, Z.; Li, N. N.; Liang, M.; Yang, B.
2015-06-01
In this study, we report on the development of a compact lamp-based vacuum ultraviolet (VUV) photoionization mass spectrometer (PIMS; hereafter referred to as VUV-PIMS) in our laboratory; it is composed of a radio frequency-powered VUV lamp, a VUV photoionizer, an ion-immigration region, and a reflection time-of-flight mass spectrometer. By utilizing the novel photoionizer consisting of a photoionization cavity and a VUV light baffle, extremely low background noise was obtained. An ultrasensitive detection limit (2σ) of 3 pptv was achieved for benzene after an acquisition time of 10 s. To examine its potential for application in real-time sample monitoring, the developed VUV-PIMS was employed for the continuous measurement of urban air for six days in Beijing, China. Strong signals of trace-level volatile organic compounds such as benzene and its alkylated derivatives were observed in the mass spectra. These initial experimental results reveal that the instrument can be used for the online monitoring of trace-level species in the atmosphere.
K-shell Photoionization of Na-like to Cl-like Ions of Mg, Si, S, Ar, and Ca
Witthoeft, M. C.; Garcia, J.; Kallman, T. R.; Bautista, M. A.; Mendoza, C.; Palmeri, P.; Quinet, P.
2010-01-01
We present R-matrix calculations of photoabsorption and photoionization cross sections across the K edge of Mg, Si, S, Ar, and Ca ions with more than 10 electrons. The calculations include the effects of radiative and Auger damping by means of an optical potential. The wave functions are constructed from single-electron. orbital bases obtained using a Thomas-Fermi-Dirac statistical model potential. Configuration interaction is considered among all states up to n = 3. The damping processes affect the resonances converging to the K-thresholds causing them to display symmetric profiles of constant width that smear the otherwise sharp edge at the photoionization threshold. These data are important for the modeling of features found in photoionized plasmas.
Vacuum-ultraviolet (VUV) photoionization of small methanol and methanol-water clusters
International Nuclear Information System (INIS)
Ahmed, Musahid; Ahmed, Musahid; Wilson, Kevin R.; Belau, Leonid; Kostko, Oleg
2008-01-01
In this work we report on the vacuum-ultraviolet (VUV) photoionization of small methanol and methanol-water clusters. Clusters of methanol with water are generated via co-expansion of the gas phase constituents in a continuous supersonic jet expansion of methanol and water seeded in Ar. The resulting clusters are investigated by single photon ionization with tunable vacuum ultraviolet synchrotron radiation and mass analyzed using reflectron mass spectrometry. Protonated methanol clusters of the form (CH3OH)nH + (n=1-12) dominate the mass spectrum below the ionization energy of the methanol monomer. With an increase in water concentration, small amounts of mixed clusters of the form (CH3OH)n(H2O)H + (n=2-11) are detected. The only unprotonated species observed in this work are the methanol monomer and dimer. Appearance energies are obtained from the photoionization efficiency (PIE) curves for CH3OH +, (CH 3OH)2 +, (CH3OH)nH + (n=1-9), and (CH 3OH)n(H2O)H + (n=2-9 ) as a function of photon energy. With an increase in the water content in the molecular beam, there is an enhancement of photoionization intensity for methanol dimer and protonated methanol monomer at threshold. These results are compared and contrasted to previous experimental observations
Galactic Winds Driven by Supernovae and Radiation Pressure: Theory and Simulations
Zhang, Dong; Davis, Shane
2018-01-01
Galactic winds are ubiquitous in most rapidly star-forming galaxies. They are crucial to the process of galaxy formation and evolution, regulating star formation, shaping the stellar mass function and the mass-metallicity relation, and enriching the intergalactic medium with metals. Although important, the physics of galactic winds is still unclear. Winds may be driven by many mechanisms including overlapping supernovae explosions, radiation pressure of starlight on dust grains, and cosmic rays. However, the growing observations of multiphase structure in galactic winds in a large number of galaxies have not been well explained by any models. In this talk I will focus on the models of supernova- and radiation-pressure-driven winds. Using the state-of-the-art numerical simulations, I will assess the relative merits of these driving mechanisms for accelerating cold and warm clouds to observed velocities, and momentum flux boost during wind propagation.
Formation of new stellar populations from gas accreted by massive young star clusters.
Li, Chengyuan; de Grijs, Richard; Deng, Licai; Geller, Aaron M; Xin, Yu; Hu, Yi; Faucher-Giguère, Claude-André
2016-01-28
Stars in clusters are thought to form in a single burst from a common progenitor cloud of molecular gas. However, massive, old 'globular' clusters--those with ages greater than ten billion years and masses several hundred thousand times that of the Sun--often harbour multiple stellar populations, indicating that more than one star-forming event occurred during their lifetimes. Colliding stellar winds from late-stage, asymptotic-giant-branch stars are often suggested to be triggers of second-generation star formation. For this to occur, the initial cluster masses need to be greater than a few million solar masses. Here we report observations of three massive relatively young star clusters (1-2 billion years old) in the Magellanic Clouds that show clear evidence of burst-like star formation that occurred a few hundred million years after their initial formation era. We show that such clusters could have accreted sufficient gas to form new stars if they had orbited in their host galaxies' gaseous disks throughout the period between their initial formation and the more recent bursts of star formation. This process may eventually give rise to the ubiquitous multiple stellar populations in globular clusters.
International Nuclear Information System (INIS)
Bourdon, A; Pasko, V P; Liu, N Y; Celestin, S; Segur, P; Marode, E
2007-01-01
This paper presents formulation of computationally efficient models of photoionization produced by non-thermal gas discharges in air based on three-group Eddington and improved Eddington (SP 3 ) approximations to the radiative transfer equation, and on effective representation of the classic integral model for photoionization in air developed by Zheleznyak et al (1982) by a set of three Helmholtz differential equations. The reported formulations represent extensions of ideas advanced recently by Segur et al (2006) and Luque et al (2007), and allow fast and accurate solution of photoionization problems at different air pressures for the range 0.1 O 2 O 2 is the partial pressure of molecular oxygen in air in units of Torr ( p O 2 = 150 Torr) at atmospheric pressure) and R in cm is an effective geometrical size of the physical system of interest. The presented formulations can be extended to other gases and gas mixtures subject to availability of related emission, absorption and photoionization coefficients. The validity of the developed models is demonstrated by performing direct comparisons of the results from these models and results obtained from the classic integral model. Specific validation comparisons are presented for a set of artificial sources of photoionizing radiation with different Gaussian dimensions, and for a realistic problem involving development of a double-headed streamer at ground pressure. The reported results demonstrate the importance of accurate definition of the boundary conditions for the photoionization production rate for the solution of second order partial differential equations involved in the Eddington, SP 3 and the Helmholtz formulations. The specific algorithms derived from the classic photoionization model of Zheleznyak et al (1982), allowing accurate calculations of boundary conditions for differential equations involved in all three new models described in this paper, are presented. It is noted that the accurate formulation of
On the Weak-Wind Problem in Massive Stars: X-Ray Spectra Reveal a Massive Hot Wind in mu Columbae
Huenemoerder, David P.; Oskinova, Lidia M.; Ignace, Richard; Waldron, Wayne L.; Todt, Helge; Hamaguchi, Kenji; Kitamoto, Shunji
2012-01-01
Mu Columbae is a prototypical weak-wind O star for which we have obtained a high-resolution X-ray spectrum with the Chandra LETG/ACIS instrument and a low-resolution spectrum with Suzaku. This allows us, for the first time, to investigate the role of X-rays on the wind structure in a bona fide weak-wind system and to determine whether there actually is a massive hot wind. The X-ray emission measure indicates that the outflow is an order of magnitude greater than that derived from UV lines and is commensurate with the nominal wind-luminosity relationship for O stars. Therefore, the "weak-wind problem"--identified from cool wind UV/optical spectra--is largely resolved by accounting for the hot wind seen in X-rays. From X-ray line profiles, Doppler shifts, and relative strengths, we find that this weak-wind star is typical of other late O dwarfs. The X-ray spectra do not suggest a magnetically confined plasma-the spectrum is soft and lines are broadened; Suzaku spectra confirm the lack of emission above 2 keV. Nor do the relative line shifts and widths suggest any wind decoupling by ions. The He-like triplets indicate that the bulk of the X-ray emission is formed rather close to the star, within five stellar radii. Our results challenge the idea that some OB stars are "weak-wind" stars that deviate from the standard wind-luminosity relationship. The wind is not weak, but it is hot and its bulk is only detectable in X-rays.
Double photoionization of helium near threshold
International Nuclear Information System (INIS)
Levin, J.C.; Armen, G.B.; Sellin, I.A.
1996-01-01
There has been substantial recent experimental interest in the ratio of double-to-single photoionization of He near threshold following several theoretical observations that earlier measurements appear to overestimate the ratio, perhaps by as much as 25%, in the first several hundred eV above threshold. The authors recent measurements are 10%-15% below these earlier results and more recent results of Doerner et al. and Samson et al. are yet another 10% lower. The authors will compare these measurement with new data, not yet analyzed, and available theory
Energy Technology Data Exchange (ETDEWEB)
Beidler, C D [Max-Planck-Institut fuer Plasmaphysik, Garching (Germany)
1991-01-01
A general expression for the magnitude of a stellarator's magnetic field, in terms of a Fourier decomposition, is too complicated to lend itself easily to analytic transport calculations. The great majority of stellarator-type devices, however, may be accurately described if one retains only those harmonics with m=0 and m=1. In the long-mean-free-path regime an analytical approximation to the particle's bounce-averaged kinetic equation can then be found. Using a numerical solution of this equation, it is possible to calculate the particle and heat fluxes due to helical-ripple transport in stellarators throughout the entire long-mean-free-path regime. 3 figs.
Simulating three-dimensional nonthermal high-energy photon emission in colliding-wind binaries
Energy Technology Data Exchange (ETDEWEB)
Reitberger, K.; Kissmann, R.; Reimer, A.; Reimer, O., E-mail: klaus.reitberger@uibk.ac.at [Institut für Astro- und Teilchenphysik and Institut für Theoretische Physik, Leopold-Franzens-Universität Innsbruck, A-6020 Innsbruck (Austria)
2014-07-01
Massive stars in binary systems have long been regarded as potential sources of high-energy γ rays. The emission is principally thought to arise in the region where the stellar winds collide and accelerate relativistic particles which subsequently emit γ rays. On the basis of a three-dimensional distribution function of high-energy particles in the wind collision region—as obtained by a numerical hydrodynamics and particle transport model—we present the computation of the three-dimensional nonthermal photon emission for a given line of sight. Anisotropic inverse Compton emission is modeled using the target radiation field of both stars. Photons from relativistic bremsstrahlung and neutral pion decay are computed on the basis of local wind plasma densities. We also consider photon-photon opacity effects due to the dense radiation fields of the stars. Results are shown for different stellar separations of a given binary system comprising of a B star and a Wolf-Rayet star. The influence of orbital orientation with respect to the line of sight is also studied by using different orbital viewing angles. For the chosen electron-proton injection ratio of 10{sup –2}, we present the ensuing photon emission in terms of two-dimensional projections maps, spectral energy distributions, and integrated photon flux values in various energy bands. Here, we find a transition from hadron-dominated to lepton-dominated high-energy emission with increasing stellar separations. In addition, we confirm findings from previous analytic modeling that the spectral energy distribution varies significantly with orbital orientation.
Alfvén wave mixing and non-JWKB waves in stellar winds
International Nuclear Information System (INIS)
Webb, G M; McKenzie, J F; Hu, Q; Zank, G P
2013-01-01
Alfvén wave mixing equations used in locally incompressible turbulence transport equations in the solar wind contain as a special case, non-Jeffreys–Wentzel–Kramers–Brouillon (non-JWKB) wave equations used in models of Alfvén wave driven winds. We discuss the canonical wave energy equation; the physical wave energy equation, and the JWKB limit of the wave interaction equations. Lagrangian and Hamiltonian variational principles for the waves are developed. Noether’s theorem is used to derive the canonical wave energy equation which is associated with the linearity symmetry of the equations. A further conservation law associated with time translation invariance of the action, applicable for steady background wind flows is also derived. In the latter case, the conserved density is the Hamiltonian density for the waves, which is distinct from the canonical wave energy density. The canonical wave energy conservation law is a special case of a wider class of conservation laws associated with Green’s theorem for the wave mixing system and the adjoint wave mixing system, which are related to Noether’s second theorem. In the sub-Alfvénic flow, inside the Alfvén point of the wind, the backward and forward waves have positive canonical energy densities, but in the super-Alfvénic flow outside the Alfvén critical point, the backward Alfvén waves are negative canonical energy waves, and the forward Alfvén waves are positive canonical energy waves. Reflection and transmission coefficients for the backward and forward waves in both the sub-Alfvénic and super-Alfvénic regions of the flow are discussed. (paper)
Revealing isomerism in sodium-water clusters: Photoionization spectra of Na(H2O)n (n = 2-90)
Dierking, Christoph W.; Zurheide, Florian; Zeuch, Thomas; Med, Jakub; Parez, Stanislav; Slavíček, Petr
2017-06-01
Soft ionization of sodium tagged polar clusters is increasingly used as a powerful technique for sizing and characterization of small aerosols with possible application, e.g., in atmospheric chemistry or combustion science. Understanding the structure and photoionization of the sodium doped clusters is critical for such applications. In this work, we report on measurements of photoionization spectra for sodium doped water clusters containing 2-90 water molecules. While most of the previous studies focused on the ionization threshold of the Na(H2O)n clusters, we provide for the first time full photoionization spectra, including the high-energy region, which are used as reference for a comparison with theory. As reported in previous work, we have seen an initial drop of the appearance ionization energy with cluster size to values of about 3.2 eV for n electron cloud. The appearance ionization energy is determined by isomers with fully solvated sodium and a highly delocalized electron cloud, while both fully and incompletely solvated isomers with localized electron clouds can contribute to the high energy part of the photoionization spectrum. Simulations at elevated temperatures show an increased abundance of isomers with low ionization energies, an entropic effect enabling size selective infrared action spectroscopy, based on near threshold photoionization of Na(H2O)n clusters. In addition, simulations of the sodium pick-up process were carried out to study the gradual formation of the hydrated electron which is the basis of the sodium-tagging sizing.
The theory of radiation driven stellar winds and the Wolf-Rayet phenomenon
International Nuclear Information System (INIS)
Abbott, D.C.
1982-01-01
The author considers the question of whether the mass loss observed from Wolf-Rayet stars can be explained by a version of wind theory which is scaled to the conditions found in the envelopes of Wolf-Rayet stars. He discusses the following topics: - The calculated radiation pressure in OB stars, and its dependence on temperature, density, and chemical composition. - A comparison between predicted and observed mass loss rates and terminal velocities for OB stars. - The applicability of the standard radiation driven wind models to Wolf-Rayet stars. - Speculations on how Wolf-Rayet stars achieve their enormous mass loss rates within the context of the radiation pressure mechanism. (Auth.)
Attosecond Time Delay in Photoionization of Noble-Gas and Halogen Atoms
Directory of Open Access Journals (Sweden)
Liang-Wen Pi
2018-02-01
Full Text Available Ultrafast processes are now accessible on the attosecond time scale due to the availability of ultrashort XUV laser pulses. Noble-gas and halogen atoms remain important targets due to their giant dipole resonance and Cooper minimum. Here, we calculate photoionization cross section, asymmetry parameter and Wigner time delay using the time-dependent local-density approximation (TDLDA, which includes the electron correlation effects. Our results are consistent with experimental data and other theoretical calculations. The asymmetry parameter provides an extra layer of access to the phase information of the photoionization processes. We find that halogen atoms bear a strong resemblance on cross section, asymmetry parameter and time delay to their noble-gas neighbors. Our predicted time delay should provide a guidance for future experiments on those atoms and related molecules.
Control of entanglement following the photoionization of trapped, hydrogen-like ions
International Nuclear Information System (INIS)
Radtke, Thomas; Fritzsche, Stephan; Surzhykov, Andrey
2005-01-01
Density matrix theory is applied to re-investigate the entanglement in the spin state of pairs of electrons following the photoionization of trapped, hydrogen-like ions. For the ionization of one out of two non-interacting atoms, in particular, we analyzed how the entanglement between the electrons is changed owing to their interaction with the radiation field. Detailed calculations on the concurrence of the final spin-state of the electrons have been performed for the photoionization of hydrogen as well as for hydrogen-like Xe 53+ and U 91+ ions. From these computations it is shown that the degree of entanglement, which is quite well preserved for neutral hydrogen, will be strongly affected by relativistic and non-dipole effects of the radiation field as the nuclear charge of the ions is increased
Double photoionization of strontium
Energy Technology Data Exchange (ETDEWEB)
Sokell, Emma; Grimm, Michael; Sheridan, Paul, E-mail: emma.sokell@ucd.i [School of Physics, University College Dublin, Belfield, Dublin 4 (Ireland)
2010-02-01
Resonant triple-differential cross-section (TDCS) measurements have been used to study the double photoionization process in strontium. Two sets of measurements were made at the photon energy of the 4p {yields} 4d resonance. The coplanar geometry was used and the fixed analyser, positioned at -90{sup 0} to the main axis of polarization of the photons, detected electrons with {approx}65% of the available excess energy. The mutual angle between the two electrons had a range just short of 90 {yields} 270{sup 0}. The TDCS exhibit unexpected lobes at a mutual angle of 180{sup 0}. Comparison with other measurements made with the same geometry but with different sharings of the available energy indicate that these TDCS all show the unexpected lobe. Some possible explanations for the lobe are considered.
Absolute photoionization cross sections of atomic oxygen
Samson, J. A. R.; Pareek, P. N.
1985-01-01
The absolute values of photoionization cross sections of atomic oxygen were measured from the ionization threshold to 120 A. An auto-ionizing resonance belonging to the 2S2P4(4P)3P(3Do, 3So) transition was observed at 479.43 A and another line at 389.97 A. The experimental data is in excellent agreement with rigorous close-coupling calculations that include electron correlations in both the initial and final states.
International Nuclear Information System (INIS)
Klein, P B; Binari, S C
2003-01-01
This review is concerned with the characterization and identification of the deep centres that cause current collapse in nitride-based field effect transistors. Photoionization spectroscopy is an optical technique that has been developed to probe the characteristics of these defects. Measured spectral dependences provide information on trap depth, lattice coupling and on the location of the defects in the device structure. The spectrum of an individual trap may also be regarded as a 'fingerprint' of the defect, allowing the trap to be followed in response to the variation of external parameters. The basis for these measurements is derived through a modelling procedure that accounts quantitatively for the light-induced drain current increase in the collapsed device. Applying the model to fit the measured variation of drain current increase with light illumination provides an estimate of the concentrations and photoionization cross-sections of the deep defects. The results of photoionization studies of GaN metal-semiconductor field effect transistors and AlGaN/GaN high electron mobility transistors (HEMTs) grown by metal-organic chemical vapour deposition (MOCVD) are presented and the conclusions regarding the nature of the deep traps responsible are discussed. Finally, recent photoionization studies of current collapse induced by short-term (several hours) bias stress in AlGaN/GaN HEMTs are described and analysed for devices grown by both MOCVD and molecular beam epitaxy. (topical review)
Apparatus for enrichment of uranium by double photoionization
International Nuclear Information System (INIS)
Laude, J.P.
1983-11-01
The present invention concerns enrichment of uranium by double photoionization. The use of a beam from a dye laser for excitation of gaseous uranium is known and the present invention concerns an apparatus of this type. The purpose of the invention is essentially to produce an apparatus having high energy efficiency. This is achieved according to the invention by using a continuous wave laser
Photoionization in negative streamers : fast computations and two propagation modes
Luque, A.; Ebert, U.M.; Montijn, C.; Hundsdorfer, W.
2007-01-01
Streamer discharges play a central role in electric breakdown of matter in pulsed electric fields, both in nature and in technology. Reliable and fast computations of the minimal model for negative streamers in simple gases such as nitrogen have recently been developed. However, photoionization was
International Nuclear Information System (INIS)
Rodriguez, R.; Gil, J.M.; Rubiano, J.G.; Florido, R.; Martel, P.; Minguez, E.
2005-01-01
Photoionization process is a subject of special importance in many areas of physics. Numerical methods must be used in order to obtain photoionization cross-sections for non-hydrogenic levels. The atomic data required to calculate them is huge so self-consistent calculations increase computing time considerably. Analytical potentials are a useful alternative because they avoid the iterative procedures typical in self-consistent models. In this work, we present a relativistic quantum calculation of photoionization cross-sections for isolated ions based on an analytical potential to obtain the required atomic data, which is valid both for hydrogenic and non-hydrogenic ions. Comparisons between our results and others obtained using either widely used analytical expressions for the cross-sections or more sophisticated calculations are done
International Nuclear Information System (INIS)
Cram, L.E.; Woods, D.T.
1982-01-01
We study the response of certain spectral signatures of stellar flares (such as Balmer line profiles and the broad-band continuum) to changes in atmospheric structure which might result from physical processes akin to those thought to occur in solar flares. While each physical process does not have a unique signature, we can show that some of the observed properties of stellar flares can be explained by a model which involves increased pressures and temperatures in the flaring stellar chromosphere. We suggest that changes in stellar flare area, both with time and with depth in the atmosphere, may play an important role in producing the observed flare spectrum
X-ray heating of laboratory photoionized plasmas at Z
Mancini, R.; Lockard, T.; Mayes, D.; Loisel, G.; Bailey, J.; Rochau, G.; Abdallah, J.; Fontes, C.; Liedahl, D.; Golovkin, I.
2017-10-01
In separate experiments performed at the Z facility of Sandia National Laboratories two different samples were employed to produce and characterize photoionized plasmas. One was a gas cell filled with neon, and the other was a thin silicon layer coated with plastic. Both samples were driven by the broadband x-ray flux produced at the collapse of a wire array z-pinch implosion. Transmission spectroscopy of a narrowband portion of the x-ray flux was used to diagnose the charge state distribution, and the electron temperature was extracted from a Li-like ion level population ratio. To interpret the temperature measurement, we performed Boltzmann kinetics and radiation-hydrodynamic simulations. We found that non-equilibrium atomic physics and the coupling of the radiation flux to the level population kinetics play a critical role in modeling the x-ray heating of photoionized plasmas. In spite of being driven by similar x-ray drives, differences of ionization and charged state distributions in the neon and silicon plasmas are reflected in the plasma heating and observed temperatures. DOE OFES Grant DE-SC0014451 and ZFSP.
ANISOTROPIC WINDS FROM CLOSE-IN EXTRASOLAR PLANETS
International Nuclear Information System (INIS)
Stone, James M.; Proga, Daniel
2009-01-01
We present two-dimensional hydrodynamic models of thermally driven winds from highly irradiated, close-in extrasolar planets. We adopt a very simple treatment of the radiative heating processes at the base of the wind, and instead focus on the differences between the properties of outflows in multidimensions in comparison to spherically symmetric models computed with the same methods. For hot (T ∼> 2 x 10 4 K) or highly ionized gas, we find that strong (supersonic) polar flows are formed above the planet surface which produce weak shocks and outflow on the night side. In comparison to a spherically symmetric wind with the same parameters, the sonic surface on the day side is much closer to the planet surface in multidimensions, and the total mass-loss rate is reduced by almost a factor of 4. We also compute the steady-state structure of interacting planetary and stellar winds. Both winds end in a termination shock, with a parabolic contact discontinuity which is draped over the planet separating the two shocked winds. The planetary wind termination shock and the sonic surface in the wind are well separated, so that the mass-loss rate from the planet is essentially unaffected. However, the confinement of the planetary wind to the small volume bounded by the contact discontinuity greatly enhances the column density close to the planet, which might be important for the interpretation of observations of absorption lines formed by gas surrounding transiting planets.
Disruption of circumstellar discs by large-scale stellar magnetic fields
ud-Doula, Asif; Owocki, Stanley P.; Kee, Nathaniel Dylan
2018-05-01
Spectropolarimetric surveys reveal that 8-10% of OBA stars harbor large-scale magnetic fields, but thus far no such fields have been detected in any classical Be stars. Motivated by this, we present here MHD simulations for how a pre-existing Keplerian disc - like that inferred to form from decretion of material from rapidly rotating Be stars - can be disrupted by a rotation-aligned stellar dipole field. For characteristic stellar and disc parameters of a near-critically rotating B2e star, we find that a polar surface field strength of just 10 G can significantly disrupt the disc, while a field of 100 G, near the observational upper limit inferred for most Be stars, completely destroys the disc over just a few days. Our parameter study shows that the efficacy of this magnetic disruption of a disc scales with the characteristic plasma beta (defined as the ratio between thermal and magnetic pressure) in the disc, but is surprisingly insensitive to other variations, e.g. in stellar rotation speed, or the mass loss rate of the star's radiatively driven wind. The disc disruption seen here for even a modest field strength suggests that the presumed formation of such Be discs by decretion of material from the star would likely be strongly inhibited by such fields; this provides an attractive explanation for why no large-scale fields are detected from such Be stars.
Photoionization of inner-shell electrons
International Nuclear Information System (INIS)
Cooper, J.W.
1975-01-01
The theory of photoionization is developed and key approximations are discussed. The formalism is fully relativistic and includes all multipoles of the radiation field, conditions that can be related at lower energies and for low Z materials. The theory can also be extended to include electron-electron correlation effects, and represents a zeroth-order approximation. Alternate ways of treating correlation effects are developed along these lines. A brief discussion is given of two methods that have been used to treat near-threshold absorption in solids and the relationship of these to the methods covered earlier is discussed. Examples are given of how well results calculated by various methods agree with experimental evidence. 5 figures, 76 references
On the photo-ionization of impurity centres in semiconductors
International Nuclear Information System (INIS)
Tomak, M.
1982-10-01
The dependence of the photo-ionization cross-section on photon energy is calculated. The impurity potential is assumed to be of the Hulthen potential type and bound state wave function is calculated variationally. The results show that, at least in some cases, the Hulthen potential may describe the impurity better than the hydrogen or delta function potentials. (author)
Photoionization in Ultraviolet Processing of Astrophysical Ice Analogs at Cryogenic Temperatures
Woon, David E.
2004-01-01
Two recent experimental studies have demonstrated that amino acids or amino acid precursors are generated when astrophysical ice analogs are subjected to ultraviolet (UV) irradiation at cryogenic temperatures. Understanding the complete phenomenology of photoprocessing is critical to elucidating chemical reaction mechanisms that can function within an ice matrix under very cold conditions. Pushing beyond the much better characterized study of photolytic dissociation of chemical bonds through electronic excitation, this work explored the ability of UV radiation present in the interstellar medium to ionize small molecules embedded in ices. Quantum chemical calculations, including bulk solvation effects, were used to study the ionization of hydrogen (H2), water, and methanol (CH3OH) bound in small clusters of water. Ionization potentials were found to be much smaller in the condensed phase than in the gas phase; even a small cluster can account for large changes in the ionization potentials in ice, as well as the known formation of an OH--H3O+ pair in the case of H2O photoionization. To gauge the impact of photoionization on subsequent grain chemistry, the reaction between OH and CO in the presence of H3O+ was studied and compared with the potential energy surface without hydronium present, which is relevant to chemistry following photolysis. The differences indicate that the reaction is somewhat more likely to proceed to products (H + CO2) in the case of photoionization.
Strong-field Photoionization of Sputtered Neutral Molecules for Molecular Depth Profiling
Willingham, D; Brenes, D. A.; Wucher, A
2009-01-01
Molecular depth profiles of an organic thin film of guanine vapor deposited onto a Ag substrate are obtained using a 40 keV C60 cluster ion beam in conjunction with time-of-flight secondary ion mass spectrometric (ToF-SIMS) detection. Strong-field, femtosecond photoionization of intact guanine molecules is used to probe the neutral component of the profile for direct comparison with the secondary ion component. The ability to simultaneously acquire secondary ions and photoionized neutral molecules reveals new fundamental information about the factors that influence the properties of the depth profile. Results show that there is an increased ionization probability for protonated molecular ions within the first 10 nm due to the generation of free protons within the sample. Moreover, there is a 50% increase in fragment ion signal relative to steady state values 25 nm before reaching the guanine/Ag interface as a result of interfacial chemical damage accumulation. An altered layer thickness of 20 nm is observed as a consequence of ion beam induced chemical mixing. In general, we show that the neutral component of a molecular depth profile using the strong-field photoionization technique can be used to elucidate the effects of variations in ionization probability on the yield of molecular ions as well as to aid in obtaining accurate information about depth dependent chemical composition that cannot be extracted from TOF-SIMS data alone. PMID:20495665
Stellar structure and evolution
International Nuclear Information System (INIS)
Kippernhahn, R.; Weigert, A.
1990-01-01
This book introduces the theory of the internal structure of stars and their evolution in time. It presents the basic physics of stellar interiors, methods for solving the underlying equations, and the most important results necessary for understanding the wide variety of stellar types and phenomena. The evolution of stars is discussed from their birth through normal evolution to possibly spectacular final stages. Chapters on stellar oscillations and rotation are included
Exploring the Dust Content of Galactic Winds with Herschel. II. Nearby Dwarf Galaxies*
McCormick, Alexander; Veilleux, Sylvain; Meléndez, Marcio; Martin, Crystal L.; Bland-Hawthorn, Joss; Cecil, Gerald; Heitsch, Fabian; Müller, Thomas; Rupke, David S. N.; Engelbracht, Chad
2018-03-01
We present results from analysis of deep Herschel Space Observatory observations of six nearby dwarf galaxies known to host galactic-scale winds. The superior far-infrared sensitivity and angular resolution of Herschel have allowed detection of cold circumgalactic dust features beyond the stellar components of the host galaxies traced by Spitzer 4.5 μm images. Comparisons of these cold dust features with ancillary data reveal an imperfect spatial correlation with the ionized gas and warm dust wind components. We find that typically ˜10-20% of the total dust mass in these galaxies resides outside of their stellar disks, but this fraction reaches ˜60% in the case of NGC 1569. This galaxy also has the largest metallicity (O/H) deficit in our sample for its stellar mass. Overall, the small number of objects in our sample precludes drawing strong conclusions on the origin of the circumgalactic dust. We detect no statistically significant trends with star formation properties of the host galaxies, as might be expected if the dust were lifted above the disk by energy inputs from on-going star formation activity. Although a case for dust entrained in a galactic wind is seen in NGC 1569, in all cases, we cannot rule out the possibility that some of the circumgalactic dust might be associated instead with gas accreted or removed from the disk by recent galaxy interaction events, or that it is part of the outer gas-rich portion of the disk that lies below the sensitivity limit of the Spitzer 4.5 μm data.
Zhu, Zhixiang; Wang, Jian; Qiu, Keqing; Liu, Chengyuan; Qi, Fei; Pan, Yang
2014-04-01
A novel vacuum ultraviolet (VUV) light source assembly (VUVLSA) for enhancing the ionization efficiency of photoionization mass spectrometer has been described. The VUVLSA composes of a Krypton lamp and a pair of disk electrodes with circular center cavities. The two interior surfaces that face the photoionization region were aluminum-coated. VUV light can be reflected back and forth in the photoionization region between the electrodes, thus the photoionization efficiency can be greatly enhanced. The performances of two different shaped electrodes, the coated double flat electrodes (DFE), and double conical electrodes, were studied. We showed that the signal amplification of coated DFE is around 4 times higher than that of uncoated electrodes without VUV light reflection. The relationship between the pressure of ionization chamber and mass signal enhancement has also been studied.
Near-Field Cosmology with Resolved Stellar Populations Around Local Volume LMC Stellar-Mass Galaxies
Carlin, Jeffrey L.; Sand, David J.; Willman, Beth; Brodie, Jean P.; Crnojevic, Denija; Forbes, Duncan; Hargis, Jonathan R.; Peter, Annika; Pucha, Ragadeepika; Romanowsky, Aaron J.; Spekkens, Kristine; Strader, Jay
2018-06-01
We discuss our ongoing observational program to comprehensively map the entire virial volumes of roughly LMC stellar mass galaxies at distances of ~2-4 Mpc. The MADCASH (Magellanic Analog Dwarf Companions And Stellar Halos) survey will deliver the first census of the dwarf satellite populations and stellar halo properties within LMC-like environments in the Local Volume. Our results will inform our understanding of the recent DES discoveries of dwarf satellites tentatively affiliated with the LMC/SMC system. This program has already yielded the discovery of the faintest known dwarf galaxy satellite of an LMC stellar-mass host beyond the Local Group, based on deep Subaru+HyperSuprimeCam imaging reaching ~2 magnitudes below its TRGB, and at least two additional candidate satellites. We will summarize the survey results and status to date, highlighting some challenges encountered and lessons learned as we process the data for this program through a prototype LSST pipeline. Our program will examine whether LMC stellar mass dwarfs have extended stellar halos, allowing us to assess the relative contributions of in-situ stars vs. merger debris to their stellar populations and halo density profiles. We outline the constraints on galaxy formation models that will be provided by our observations of low-mass galaxy halos and their satellites.
Molecular photoionization using the complex Kohn variational method
International Nuclear Information System (INIS)
Lynch, D.L.; Schneider, B.I.
1992-01-01
We have applied the complex Kohn variational method to the study of molecular-photoionization processes. This requires electron-ion scattering calculations enforcing incoming boundary conditions. The sensitivity of these results to the choice of the cutoff function in the Kohn method has been studied and we have demonstrated that a simple matching of the irregular function to a linear combination of regular functions produces accurate scattering phase shifts
Winds of Massive Magnetic Stars: Interacting Fields and Flow
Daley-Yates, S.; Stevens, I. R.
2018-01-01
We present results of 3D numerical simulations of magnetically confined, radiatively driven stellar winds of massive stars, conducted using the astrophysical MHD code Pluto, with a focus on understanding the rotational variability of radio and sub-mm emission. Radiative driving is implemented according to the Castor, Abbott and Klein theory of radiatively driven winds. Many magnetic massive stars posses a magnetic axis which is inclined with respect to the rotational axis. This misalignment leads to a complex wind structure as magnetic confinement, centrifugal acceleration and radiative driving act to channel the circumstellar plasma into a warped disk whose observable properties should be apparent in multiple wavelengths. This structure is analysed to calculate free-free thermal radio emission and determine the characteristic intensity maps and radio light curves.
Supernova blast wave within a stellar cluster outflow
Rodríguez-Ramírez, J. C.; Raga, A. C.; Velázquez, P. F.; Rodríguez-González, A.; Toledo-Roy, J. C.
2014-11-01
In this paper, we develop a semi-analytic model of a supernova which goes off in the centre of a stellar cluster. The supernova remnant interacts with a stratified, pre-existent outflow produced by the winds of the cluster stars. We compare our semi-analytic model with numerical simulations using the spherically symmetric Euler equations with appropriate mass and energy source terms. We find good agreement between these two approaches, and we find that for typical parameters the blast wave is likely to reach the Taylor-Sedov regime outside the cluster radius. We also calculate the predicted X-ray luminosity of the flow as a function of time, and we obtain its dependence on the outer radius and the number of stars of the cluster.
International Nuclear Information System (INIS)
Moroz, P.E.
1997-09-01
A new stellarator configuration, the Double-Helix Stellarator (DHS), is introduced. This novel configuration features a double-helix center post as the only helical element of the stellarator coil system. The DHS configuration has many unique characteristics. One of them is the extreme low plasma aspect ratio, A ∼ 1--1.2. Other advantages include a high enclosed volume, appreciable rotational transform, and a possibility of extreme-high-β MHD equilibria. Moreover, the DHS features improved transport characteristics caused by the absence of the magnetic field ripple on the outboard of the torus. Compactness, simplicity and modularity of the coil system add to the DHS advantages for fusion applications
The Role of Stellar Feedback on the Structure of the ISM and Star Formation in Galaxies
Grisdale, Kearn Michael
2017-08-01
Stellar feedback refers to the injection of energy, momentum and mass into the interstellar medium (ISM) by massive stars. This feedback owes to a combination of ionising radiation, radiation pressure, stellar winds and supernovae and is likely responsible both for the inefficiency of star formation in galaxies, and the observed super-sonic turbulence of the ISM. In this thesis, I study how stellar feedback shapes the ISM thereby regulating galaxy evolution. In particular, I focus on three key questions: (i) How does stellar feedback shape the gas density distribution of the ISM? (ii) How does feedback change or influence the distribution of the kinetic energy in the ISM? and (iii) What role does feedback play in determining the star formation efficiency of giant molecular clouds (GMCs)? To answer these questions, I run high resolution (Deltax 4.6 pc) numerical simulations of three isolated galaxies, both with and without stellar feedback. I compare these simulations to observations of six galaxies from The HI Nearby Galaxy Survey (THINGS) using power spectra, and I use clump finding techniques to identify GMCs in my simulations and calculate their properties. I find that the kinetic energy power spectra in stellar feedback- regulated galaxies, regardless of the galaxy's mass and size, show scalings in excellent agreement with supersonic turbulence on scales below the thickness of the HI layer. I show that feedback influences the gas density field, and drives gas turbulence, up to large (kiloparsec) scales. This is in stark contrast to the density fields generated by large-scale gravity-only driven turbulence (i.e. without stellar feedback). Simulations with stellar feedback are able to reproduce the internal properties of GMCs such as: mass, size and velocity dispersion. Finally, I demonstrate that my simulations naturally reproduce the observed scatter (3.5-4 dex) in the star formation efficiency per free-fall time of GMCs, despite only employing a simple Schmidt
International Nuclear Information System (INIS)
Hollauer, E.; Nascimento, M.A.C.
1985-01-01
The photoionization cross-section and dynamic polarizability for lithium atom are calculated using a discrete basis set to represent both the bound and the continuum-states of the atom, to construct an approximation to the dynamic polarizability. From the imaginary part of the complex dynamic polarizability one extracts the photoionization cross-section and from its real part the dynamic polarizability. The results are in good agreement with the experiments and other more elaborate calculations (Author) [pt
Azoury, Doron; Krüger, Michael; Orenstein, Gal; Larsson, Henrik R; Bauch, Sebastian; Bruner, Barry D; Dudovich, Nirit
2017-11-13
Single-photon ionization is one of the most fundamental light matter interactions in nature, serving as a universal probe of the quantum state of matter. By probing the emitted electron, one can decode the full dynamics of the interaction. When photo-ionization is evolving in the presence of a strong laser field, the fundamental properties of the mechanism can be signicantly altered. Here we demonstrate how the liberated electron can perform a self-probing measurement of such interaction with attosecond precision. Extreme ultraviolet attosecond pulses initiate an electron wavepacket by photo-ionization, a strong infrared field controls its motion, and finally electron-ion collision maps it into re-emission of attosecond radiation bursts. Our measurements resolve the internal clock provided by the self-probing mechanism, obtaining a direct insight into the build-up of photo-ionization in the presence of the strong laser field.
International Nuclear Information System (INIS)
Zhou, B.; Lin, C.D.
1994-01-01
Photoionization cross sections from the metastable state (1s2s) 1 Se of the He atom for photon energies between the He + (N=2) and (N=3) thresholds are calculated using the hyperspherical close-coupling method. The calculated spectra are convoluted with an energy resolution of 5.4 meV and are compared with the spectra for photoionization from the ground state. It is found that among the four possible outgoing channels, the 1sεp channel, which is the dominant channel for photoionization from the ground state, makes negligible contributions to the total cross sections for photoionization from the metastable state. As a result, the propensity rule derived from the ground-state photoionization no longer applies and more series of the doubly excited states are populated with significant spectral intensity in photoionization from the metastable state. Photoionization cross sections from the metastable (1s2s) 3 Se state are also calculated and analyzed
Magnetic surfaces and localized perturbations in the Wendelstein VII-A stellarator
International Nuclear Information System (INIS)
Wobig, H.
1986-09-01
The critical dependence of plasma confinement in low-shear stellarators, such as Wendelstein VII-A, on the external rotational transform can be explained on the basis of magnetic surface destruction. External symmetry-breaking perturbations generate islands on the low order rational magnetic surfaces. The islands are largest at t=1/2 and t=1/3. Confinement is optimum in close proximity to these values. In order to study the structure of surfaces under the influence of perturbations, a mapping procedure is used instead of field line integration. It is found that the neighbourhood of low- order rational surfaces is particularly robust against surface destruction. The reason is that in this vicinity only rational surfaces with large m and n exist (t=m/n). On these surfaces the external perturbation only generates small islands. In W VII-A the current leads to the helical windings are one symmetry- breaking perturbation, and there might also be others. It is possible to avoid field errors of this kind in future stellarators. (orig.)
Carlin, Jeffrey L.; Sand, David J.; Willman, Beth; Brodie, Jean P.; Crnojevic, Denija; Peter, Annika; Price, Paul A.; Romanowsky, Aaron J.; Spekkens, Kristine; Strader, Jay
2017-01-01
We discuss the first results of our observational program to comprehensively map nearly the entire virial volumes of roughly LMC stellar mass galaxies at distances of ~2-4 Mpc. The MADCASH (Magellanic Analog Dwarf Companions And Stellar Halos) survey will deliver the first census of the dwarf satellite populations and stellar halo properties within LMC-like environments in the Local Volume. These will inform our understanding of the recent DES discoveries of dwarf satellites tentatively affiliated with the LMC/SMC system. We will detail our discovery of the faintest known dwarf galaxy satellite of an LMC stellar-mass host beyond the Local Group, based on deep Subaru+HyperSuprimeCam imaging reaching ~2 magnitudes below its TRGB. We will summarize the survey results and status to date, highlighting some challenges encountered and lessons learned as we process the data for this program through a prototype LSST pipeline. Our program will examine whether LMC stellar mass dwarfs have extended stellar halos, allowing us to assess the relative contributions of in-situ stars vs. merger debris to their stellar populations and halo density profiles. We outline the constraints on galaxy formation models that will be provided by our observations of low-mass galaxy halos and their satellites.
Population of the 3P2,1,0 fine-structure states in the 3s and 3p photoionization of atomic chlorine
International Nuclear Information System (INIS)
Krause, M.O.; Caldwell, C.D.; Whitfield, S.B.; de Lange, C.A.; van der Meulen, P.
1993-01-01
In a high-resolution photoelectron-spectrometry study of the photoionization of chlorine atoms in both the 3s and 3p subshells, we were able to resolve contributions from ionic states with specific J values and measure the relative populations of these fine-structure components. Our photoelectron spectra, recorded at hν=29.2 eV, give ratios of 3 P 2 : 3 P 1 : 3 P 0 =100:40.59.5 for 3p photoionization and 3 P 2 : 3 P 1 =100:31 for 3s photoionization. While the results for 3p ionization are in accord with predictions based on a simple geometric analysis, the contribution of the 3 P 1 state in 3s photoionization is larger than that predicted by this simple model. The geometric predictions are also compared with results from a similar measurement of the population of the 4p -1 ( 3 P J ) states produced in the 4p ionization of Br and with earlier work on the production of 3 D 2,1,0 states in d-shell photoionization of Cu and Ag
FITspec: A New Algorithm for the Automated Fit of Synthetic Stellar Spectra for OB Stars
Fierro-Santillán, Celia R.; Zsargó, Janos; Klapp, Jaime; Díaz-Azuara, Santiago A.; Arrieta, Anabel; Arias, Lorena; Sigalotti, Leonardo Di G.
2018-06-01
In this paper we describe the FITspec code, a data mining tool for the automatic fitting of synthetic stellar spectra. The program uses a database of 27,000 CMFGEN models of stellar atmospheres arranged in a six-dimensional (6D) space, where each dimension corresponds to one model parameter. From these models a library of 2,835,000 synthetic spectra were generated covering the ultraviolet, optical, and infrared regions of the electromagnetic spectrum. Using FITspec we adjust the effective temperature and the surface gravity. From the 6D array we also get the luminosity, the metallicity, and three parameters for the stellar wind: the terminal velocity ({v}∞ ), the β exponent of the velocity law, and the clumping filling factor (F cl). Finally, the projected rotational velocity (v\\cdot \\sin i) can be obtained from the library of stellar spectra. Validation of the algorithm was performed by analyzing the spectra of a sample of eight O-type stars taken from the IACOB spectroscopic survey of Northern Galactic OB stars. The spectral lines used for the adjustment of the analyzed stars are reproduced with good accuracy. In particular, the effective temperatures calculated with the FITspec are in good agreement with those derived from spectral type and other calibrations for the same stars. The stellar luminosities and projected rotational velocities are also in good agreement with previous quantitative spectroscopic analyses in the literature. An important advantage of FITspec over traditional codes is that the time required for spectral analyses is reduced from months to a few hours.
Photoionization of image states around metallic nanotubes
Energy Technology Data Exchange (ETDEWEB)
Segui, Silvina; Arista, Nestor R; Gervasoni, Juana L [Centro Atomico Bariloche (CNEA) 8400, Rio Negro (Argentina); Bocan, Gisela A, E-mail: segui@cab.cnea.gov.a, E-mail: gbocan@iafe.uba.a, E-mail: arista@cab.cnea.gov.a, E-mail: gervason@cab.cnea.gov.a [Institute de AstronomIa y Fisica del Espacio, CC 67, Sue 28, 1428, Ciudad Universitaria, Buenos Aires (Argentina)
2009-11-01
In this work we study a theoretical approach to the ionization of electrons bound in an image state around a metallic nanotube by the impact of photons. In a close analogy to the already studied case of ionization by electron impact [1], we calculate and analyze photoionization cross sections of tubular image states [2] within a first Born approximation. We consider various situations, including different energies and polarizations of the incident photon, ejection directions of the outgoing electron, and angular momenta of the image state.
Near threshold double photoionization of rare gases
International Nuclear Information System (INIS)
Huetz, A.; Selles, P.; Waymel, D.; Mazeau, J.
1992-01-01
Double photoionization experiments using a helium discharge lamp have been performed for the outermost shells of krypton and xenon. For the first time both the energies and the angles of the two outgoing electrons have been selected, allowing measurements of the triple differential cross sections. These are expressed as products of two factors, the first factor accounts for symmetry and rotation and the second for angular correlation. The latter is then extracted from the experiments and compared with theoretical predictions deduced from the Wannier model. (Author)
Photoionization mass spectrometer for studies of flame chemistry with a synchrotron light source
International Nuclear Information System (INIS)
Cool, Terrill A.; McIlroy, Andrew; Qi, Fei; Westmoreland, Phillip R.; Poisson, Lionel; Peterka, Darcy S.; Ahmed, Musahid
2005-01-01
A flame-sampling molecular-beam photoionization mass spectrometer, recently designed and constructed for use with a synchrotron-radiation light source, provides significant improvements over previous molecular-beam mass spectrometers that have employed either electron-impact ionization or vacuum ultraviolet laser photoionization. These include superior signal-to-noise ratio, soft ionization, and photon energies easily and precisely tunable [E/ΔE(FWHM)≅250-400] over the 7.8-17-eV range required for quantitative measurements of the concentrations and isomeric compositions of flame species. Mass resolution of the time-of-flight mass spectrometer is m/Δm=400 and sensitivity reaches ppm levels. The design of the instrument and its advantages for studies of flame chemistry are discussed
Studies of photoionization in liquids using a laser two-photon ionization conductivity technique
International Nuclear Information System (INIS)
Siomos, K.; Christophorou, L.G.
1981-01-01
One-photon ionization studies of solute molecules in a liquid medium are limited by the absorption of the host medium. A laser two-photon ionization (TPI) technique using a frequency tunable dye laser has been developed, whereby the photoionization threshold of a solute molecule was determined from the induced conductivity in the liquid medium under study due to electron-ion pair formation via two-photon ionization of the solute. The two-photon induced electron-ion current is measured as a function of the laser wavelength, lambda/sub laser/. In this paper, results are reported and discussed on the photoionization of N,N,N',N'-tetramethyl-p-phenylenediamine (TMPD), pyrene and fluoranthene in liquid n-pentane
Pan, Yang; Hu, Yonghua; Wang, Jian; Ye, Lili; Liu, Chengyuan; Zhu, Zhixiang
2013-12-17
A newly developed, qualitative and quantitative method based on tunable synchrotron radiation vacuum ultraviolet photoionization time-of-flight mass spectrometry (SR-VUV-PI-TOFMS) and photoionization efficiency (PIE) curve simulation was applied for the online analysis of isomers and isobaric compounds in the gas phase of mainstream cigarette smoke. After blocking the particulate phase components by the Cambridge filter pad, a puff of fresh gas-phase cigarette smoke was immediately introduced into a vacuum ionization chamber through a heated capillary, then was photoionized, and analyzed by a TOF mass spectrometer. The PIE curves for the mass peaks up to m/z = 106 were measured between 8.0 and 10.7 eV. Some components could be directly identified by their discriminated ionization energies (IEs) on the PIE curve. By simulating the PIE curve with the sum of scaled absolute photoionization cross sections (PICSs), complex isomeric/isobaric compounds along with their mole fractions could be obtained when the best-fitting was realized between experimental and simulated PIE curves. A series of reported toxic compounds for quantification, such as 1,3-butadiene (m/z = 54), 1,3-cyclopentadiene (m/z = 66), benzene (m/z = 78), xylene (m/z = 106), 2-propenal (m/z = 56), acetone and propanal (m/z = 58), crotonaldehyde (m/z = 70), furan and isoprene (m/z = 68), were all found to have other isomers and/or isobaric compounds with considerable abundances. Some isomers have never been reported previously in cigarette smoke, like C5H6 isomers 1-penten-3-yne, 3-penten-1-yne, and 1-penten-4-yne at m/z = 66. Isomeric/isobaric compounds characterization for the mass peaks and mole fraction calculations were discussed in detail below 10.7 eV, an energy value covering several conventional used VUV light sources.
Effect of core polarizability on photoionization cross-section calculations.
Kirkpatrick, R. C.
1972-01-01
Demonstration of the importance of core polarizability in a case where cancellation is only moderate, with suggestion of an improvement to the scaled Thomas-Fermi (STF) wave functions of Stewart and Rotenberg (1965). The inclusion of dipole polarizability of the core for argon is shown to substantially improve the agreement between the theoretical and experimental photoionization cross sections for the ground-state configuration.
Soft x-ray photoionization of atoms and molecules
International Nuclear Information System (INIS)
Svensson, Svante
2005-01-01
A review of resonant and non-resonant electron spectroscopy on atoms and molecules at third generation synchrotron radiation facilities is given. The high brilliance of the soft x-ray radiation has made possible new types of experiments giving information on the fundamental behaviour of photoionization. The relevance of Einstein's photoelectric law, and notably the question of when electron energies disperse or do not disperse with the photon energy, is given special attention
Schneider, F.R.N.; Izzard, R.G.; de Mink, S.E.; Langer, N.; Stolte, A.; de Koter, A.; Gvaramadze, V.V.; Huβman, B.; Liermann, A.; Sana, H.
2014-01-01
Massive stars rapidly change their masses through strong stellar winds and mass transfer in binary systems. The latter aspect is important for populations of massive stars as more than 70% of all O stars are expected to interact with a binary companion during their lifetime. We show that such mass
Revealing isomerism in sodium-water clusters: Photoionization spectra of Na(H2O)n (n = 2-90).
Dierking, Christoph W; Zurheide, Florian; Zeuch, Thomas; Med, Jakub; Parez, Stanislav; Slavíček, Petr
2017-06-28
Soft ionization of sodium tagged polar clusters is increasingly used as a powerful technique for sizing and characterization of small aerosols with possible application, e.g., in atmospheric chemistry or combustion science. Understanding the structure and photoionization of the sodium doped clusters is critical for such applications. In this work, we report on measurements of photoionization spectra for sodium doped water clusters containing 2-90 water molecules. While most of the previous studies focused on the ionization threshold of the Na(H 2 O) n clusters, we provide for the first time full photoionization spectra, including the high-energy region, which are used as reference for a comparison with theory. As reported in previous work, we have seen an initial drop of the appearance ionization energy with cluster size to values of about 3.2 eV for nphotoionization spectrum. Simulations at elevated temperatures show an increased abundance of isomers with low ionization energies, an entropic effect enabling size selective infrared action spectroscopy, based on near threshold photoionization of Na(H 2 O) n clusters. In addition, simulations of the sodium pick-up process were carried out to study the gradual formation of the hydrated electron which is the basis of the sodium-tagging sizing.
International Nuclear Information System (INIS)
Desmazières, Bernard; Legros, Véronique; Giuliani, Alexandre; Buchmann, William
2014-01-01
Graphical abstract: Atmospheric pressure photoIonization mass spectra of synthetic oligomers were recorded in the negative mode by varying the photon energy using synchrotron radiation. Photon energy required for an efficient ionization of the polymer was correlated to ionization potential of the solvent (for example 9.4 eV for tetrahydrofuran). -- Highlights: •Atmospheric pressure photoionization was performed using synchrotron radiation. •Photoionization of oligomers in THF with 10% CH 2 Cl 2 produces intact [M + Cl] − ions. •The photon energy required corresponds to ionization potential of the solvent. •Polymer distributions depend on source parameters such T °C and applied voltages. •Liquid chromatography was coupled to MS using an APPI interface for polymer analysis. -- Abstract: Atmospheric pressure photoionization (APPI) followed by mass spectrometric detection was used to ionize a variety of polymers: polyethylene glycol, polymethyl methacrylate, polystyrene, and polysiloxane. In most cases, whatever the polymer or the solvent used (dichloromethane, tetrahydrofuran, hexane, acetone or toluene), only negative ion mode produced intact ions such as chlorinated adducts, with no or few fragmentations, in contrast to the positive ion mode that frequently led to important in-source fragmentations. In addition, it was shown that optimal detection of polymer distributions require a fine tuning of other source parameters such as temperature and ion transfer voltage. Series of mass spectra were recorded in the negative mode, in various solvents (dichloromethane, tetrahydrofuran, hexane, toluene, and acetone), by varying the photon energy from 8 eV up to 10.6 eV using synchrotron radiation. To these solvents, addition of a classical APPI dopant (toluene or acetone) was not necessary. Courtesy of the synchrotron radiation, it was demonstrated that the photon energy required for an efficient ionization of the polymer was correlated to the ionization energy
Energy Technology Data Exchange (ETDEWEB)
Desmazières, Bernard [Global Bioenergies, 5 rue Henri Desbruyeres, 91030 Evry (France); Legros, Véronique [CNRS, UMR8587, Université d’Evry-Val-d’Essonne, Laboratoire Analyse et Modélisation pour la Biologie et l’Environnement, F-91025 Evry (France); Giuliani, Alexandre [Synchrotron SOLEIL, L’Orme des Merisiers, Saint-Aubin, 91192 Gif-sur-Yvette (France); UAR1008, CEPIA, INRA, Rue de la Geraudiere, F-44316 Nantes (France); Buchmann, William, E-mail: william.buchmann@univ-evry.fr [CNRS, UMR8587, Université d’Evry-Val-d’Essonne, Laboratoire Analyse et Modélisation pour la Biologie et l’Environnement, F-91025 Evry (France)
2014-01-15
Graphical abstract: Atmospheric pressure photoIonization mass spectra of synthetic oligomers were recorded in the negative mode by varying the photon energy using synchrotron radiation. Photon energy required for an efficient ionization of the polymer was correlated to ionization potential of the solvent (for example 9.4 eV for tetrahydrofuran). -- Highlights: •Atmospheric pressure photoionization was performed using synchrotron radiation. •Photoionization of oligomers in THF with 10% CH{sub 2}Cl{sub 2} produces intact [M + Cl]{sup −} ions. •The photon energy required corresponds to ionization potential of the solvent. •Polymer distributions depend on source parameters such T °C and applied voltages. •Liquid chromatography was coupled to MS using an APPI interface for polymer analysis. -- Abstract: Atmospheric pressure photoionization (APPI) followed by mass spectrometric detection was used to ionize a variety of polymers: polyethylene glycol, polymethyl methacrylate, polystyrene, and polysiloxane. In most cases, whatever the polymer or the solvent used (dichloromethane, tetrahydrofuran, hexane, acetone or toluene), only negative ion mode produced intact ions such as chlorinated adducts, with no or few fragmentations, in contrast to the positive ion mode that frequently led to important in-source fragmentations. In addition, it was shown that optimal detection of polymer distributions require a fine tuning of other source parameters such as temperature and ion transfer voltage. Series of mass spectra were recorded in the negative mode, in various solvents (dichloromethane, tetrahydrofuran, hexane, toluene, and acetone), by varying the photon energy from 8 eV up to 10.6 eV using synchrotron radiation. To these solvents, addition of a classical APPI dopant (toluene or acetone) was not necessary. Courtesy of the synchrotron radiation, it was demonstrated that the photon energy required for an efficient ionization of the polymer was correlated to the
International Nuclear Information System (INIS)
Beidler, C.D.; Hitchon, W.N.G.
1993-08-01
Calculations of the neoclassical transport rates due to particles trapped in the helical ripples of a stellarator's magnetic field are carried out, based on solutions of the bounce-averaged kinetic equation. These calculations employ a model for the magnetic field strength, B, which is an accurate approximation to the actual B for a wide variety of stellarator-type devices, among which are Helical-Axis Advanced Stellarators (Helias) as well as conventional stellarators and torsatrons. Comparisons are carried out in which it is shown that the Helias concept leads to significant reductions in neoclassical transport rates throughout the entire long-mean-free-path regime, with the reduction being particularly dramatic in the ν -1 regime. These findings are confirmed by numerical simulations. Further, it is shown that the behavior of deeply trapped particles in Helias can be fundamentally different from that in classical stellarator/torsatrons; as a consequence, the beneficial effects of a radial electric field on the transport make themselves felt at lower collision frequency than is usual. (orig.)
Convection and stellar oscillations
DEFF Research Database (Denmark)
Aarslev, Magnus Johan
2017-01-01
for asteroseismology, because of the challenges inherent in modelling turbulent convection in 1D stellar models. As a result of oversimplifying the physics near the surface, theoretical calculations systematically overestimate the oscillation frequencies. This has become known as the asteroseismic surface effect. Due...... to lacking better options, this frequency difference is typically corrected for with ad-hoc formulae. The topic of this thesis is the improvement of 1D stellar convection models and the effects this has on asteroseismic properties. The source of improvements is 3D simulations of radiation...... atmospheres to replace the outer layers of stellar models. The additional turbulent pressure and asymmetrical opacity effects in the atmosphere model, compared to convection in stellar evolution models, serve to expand the atmosphere. The enlarged acoustic cavity lowers the pulsation frequencies bringing them...
Stellarator Research Opportunities: A report of the National Stellarator Coordinating Committee
Energy Technology Data Exchange (ETDEWEB)
Gates, David A. [Princeton Plasma Physics Lab. (PPPL), Princeton, NJ (United States); Anderson, David [University of Wisconsin-Madison
2017-06-01
This document is the product of a stellarator community workshop, organized by the National Stellarator Coordinating Committee and referred to as Stellcon, that was held in Cambridge, Massachusetts in February 2016, hosted by MIT. The workshop was widely advertised, and was attended by 40 scientists from 12 different institutions including national labs, universities and private industry, as well as a representative from the Department of Energy. The final section of this document describes areas of community wide consensus that were developed as a result of the discussions held at that workshop. Areas where further study would be helpful to generate a consensus path forward for the US stellarator program are also discussed. The program outlined in this document is directly responsive to many of the strategic priorities of FES as articulated in “Fusion Energy Sciences: A Ten-Year Perspective (2015-2025)” [2]. The natural disruption immunity of the stellarator directly addresses “Elimination of transient events that can be deleterious to toroidal fusion plasma confinement devices” an area of critical importance for the U.S. fusion energy sciences enterprise over the next decade. Another critical area of research “Strengthening our partnerships with international research facilities,” is being significantly advanced on the W7-X stellarator in Germany and serves as a test-bed for development of successful international collaboration on ITER. This report also outlines how materials science as it relates to plasma and fusion sciences, another critical research area, can be carried out effectively in a stellarator. Additionally, significant advances along two of the Research Directions outlined in the report; “Burning Plasma Science: Foundations - Next-generation research capabilities”, and “Burning Plasma Science: Long pulse - Sustainment of Long-Pulse Plasma Equilibria” are proposed.
Stellarator Research Opportunities: A Report of the National Stellarator Coordinating Committee
Gates, D. A.; Anderson, D.; Anderson, S.; Zarnstorff, M.; Spong, D. A.; Weitzner, H.; Neilson, G. H.; Ruzic, D.; Andruczyk, D.; Harris, J. H.; Mynick, H.; Hegna, C. C.; Schmitz, O.; Talmadge, J. N.; Curreli, D.; Maurer, D.; Boozer, A. H.; Knowlton, S.; Allain, J. P.; Ennis, D.; Wurden, G.; Reiman, A.; Lore, J. D.; Landreman, M.; Freidberg, J. P.; Hudson, S. R.; Porkolab, M.; Demers, D.; Terry, J.; Edlund, E.; Lazerson, S. A.; Pablant, N.; Fonck, R.; Volpe, F.; Canik, J.; Granetz, R.; Ware, A.; Hanson, J. D.; Kumar, S.; Deng, C.; Likin, K.; Cerfon, A.; Ram, A.; Hassam, A.; Prager, S.; Paz-Soldan, C.; Pueschel, M. J.; Joseph, I.; Glasser, A. H.
2018-02-01
This document is the product of a stellarator community workshop, organized by the National Stellarator Coordinating Committee and referred to as Stellcon, that was held in Cambridge, Massachusetts in February 2016, hosted by MIT. The workshop was widely advertised, and was attended by 40 scientists from 12 different institutions including national labs, universities and private industry, as well as a representative from the Department of Energy. The final section of this document describes areas of community wide consensus that were developed as a result of the discussions held at that workshop. Areas where further study would be helpful to generate a consensus path forward for the US stellarator program are also discussed. The program outlined in this document is directly responsive to many of the strategic priorities of FES as articulated in "Fusion Energy Sciences: A Ten-Year Perspective (2015-2025)" [1]. The natural disruption immunity of the stellarator directly addresses "Elimination of transient events that can be deleterious to toroidal fusion plasma confinement devices" an area of critical importance for the US fusion energy sciences enterprise over the next decade. Another critical area of research "Strengthening our partnerships with international research facilities," is being significantly advanced on the W7-X stellarator in Germany and serves as a test-bed for development of successful international collaboration on ITER. This report also outlines how materials science as it relates to plasma and fusion sciences, another critical research area, can be carried out effectively in a stellarator. Additionally, significant advances along two of the Research Directions outlined in the report; "Burning Plasma Science: Foundations - Next-generation research capabilities", and "Burning Plasma Science: Long pulse - Sustainment of Long-Pulse Plasma Equilibria" are proposed.
Habitability in different Milky Way stellar environments: a stellar interaction dynamical approach.
Jiménez-Torres, Juan J; Pichardo, Bárbara; Lake, George; Segura, Antígona
2013-05-01
Every Galactic environment is characterized by a stellar density and a velocity dispersion. With this information from literature, we simulated flyby encounters for several Galactic regions, numerically calculating stellar trajectories as well as orbits for particles in disks; our aim was to understand the effect of typical stellar flybys on planetary (debris) disks in the Milky Way Galaxy. For the solar neighborhood, we examined nearby stars with known distance, proper motions, and radial velocities. We found occurrence of a disturbing impact to the solar planetary disk within the next 8 Myr to be highly unlikely; perturbations to the Oort cloud seem unlikely as well. Current knowledge of the full phase space of stars in the solar neighborhood, however, is rather poor; thus we cannot rule out the existence of a star that is more likely to approach than those for which we have complete kinematic information. We studied the effect of stellar encounters on planetary orbits within the habitable zones of stars in more crowded stellar environments, such as stellar clusters. We found that in open clusters habitable zones are not readily disrupted; this is true if they evaporate in less than 10(8) yr. For older clusters the results may not be the same. We specifically studied the case of Messier 67, one of the oldest open clusters known, and show the effect of this environment on debris disks. We also considered the conditions in globular clusters, the Galactic nucleus, and the Galactic bulge-bar. We calculated the probability of whether Oort clouds exist in these Galactic environments.
Relativistic effects in photoionization time delay near the Cooper minimum of noble-gas atoms
Saha, Soumyajit; Mandal, Ankur; Jose, Jobin; Varma, Hari R.; Deshmukh, P. C.; Kheifets, A. S.; Dolmatov, V. K.; Manson, S. T.
2014-11-01
Time delay of photoemission from valence n s , n p3 /2 , and n p1 /2 subshells of noble-gas atoms is theoretically scrutinized within the framework of the dipole relativistic random phase approximation. The focus is on the variation of time delay in the vicinity of the Cooper minima in photoionization of the outer subshells of neon, argon, krypton, and xenon, where the corresponding dipole matrix element changes its sign while passing through a node. It is revealed that the presence of the Cooper minimum in one photoionization channel has a strong effect on time delay in other channels. This is shown to be due to interchannel coupling.
Effects of stellar evolution and ionizing radiation on the environments of massive stars
Mackey, J.; Langer, N.; Mohamed, S.; Gvaramadze, V. V.; Neilson, H. R.; Meyer, D. M.-A.
2014-09-01
We discuss two important effects for the astrospheres of runaway stars: the propagation of ionizing photons far beyond the astropause, and the rapid evolution of massive stars (and their winds) near the end of their lives. Hot stars emit ionizing photons with associated photoheating that has a significant dynamical effect on their surroundings. 3-D simulations show that H ii regions around runaway O stars drive expanding conical shells and leave underdense wakes in the medium they pass through. For late O stars this feedback to the interstellar medium is more important than that from stellar winds. Late in life, O stars evolve to cool red supergiants more rapidly than their environment can react, producing transient circumstellar structures such as double bow shocks. This provides an explanation for the bow shock and linear bar-shaped structure observed around Betelgeuse.
Colliding winds: Interaction regions with strong heat conduction
International Nuclear Information System (INIS)
Imamura, J.N.; Chevalier, R.A.
1984-01-01
The interaction of fast stellar wind with a slower wind from previous mass loss gives rise to a region of hot, shocked gas. We obtain self-similar solutions for the interaction region under the assumptions of constant mass loss rate and wind velocity for the two winds, conversion of energy in the shock region, and either isothermal electrons and adiabatic ions or isothermal electrons ad ions in the shocked region. The isothermal assumption is intended to show the effects of strog heat conduction. The solutions have no heat conduction through the shock waves and assume that the electron and ion temperatures are equilibriated in the shock waves. The one-temperature isothermal solutions have nearly constant density through the shocked region, while the two-temperature solutions are intermediate between the one-temperature adiabatic and isothermal solutions. In the two-temperature solutions, the ion temperature goes to zero at the point where the gas comoves with the shocked region and the density peaks at this point. The solution may qualitatively describe the effects of heat conduction on interaction regions in the solar wind. It will be important to determine whether the assumption of no thermal waves outside the shocked region applies to shock waves in the solar wind
The “Building Blocks” of Stellar Halos
Directory of Open Access Journals (Sweden)
Kyle A. Oman
2017-08-01
Full Text Available The stellar halos of galaxies encode their accretion histories. In particular, the median metallicity of a halo is determined primarily by the mass of the most massive accreted object. We use hydrodynamical cosmological simulations from the apostle project to study the connection between the stellar mass, the metallicity distribution, and the stellar age distribution of a halo and the identity of its most massive progenitor. We find that the stellar populations in an accreted halo typically resemble the old stellar populations in a present-day dwarf galaxy with a stellar mass ∼0.2–0.5 dex greater than that of the stellar halo. This suggests that had they not been accreted, the primary progenitors of stellar halos would have evolved to resemble typical nearby dwarf irregulars.
Constraining the Stellar Mass Function in the Galactic Center via Mass Loss from Stellar Collisions
Directory of Open Access Journals (Sweden)
Douglas Rubin
2011-01-01
Full Text Available The dense concentration of stars and high-velocity dispersions in the Galactic center imply that stellar collisions frequently occur. Stellar collisions could therefore result in significant mass loss rates. We calculate the amount of stellar mass lost due to indirect and direct stellar collisions and find its dependence on the present-day mass function of stars. We find that the total mass loss rate in the Galactic center due to stellar collisions is sensitive to the present-day mass function adopted. We use the observed diffuse X-ray luminosity in the Galactic center to preclude any present-day mass functions that result in mass loss rates >10-5M⨀yr−1 in the vicinity of ~1″. For present-day mass functions of the form, dN/dM∝M-α, we constrain the present-day mass function to have a minimum stellar mass ≲7M⨀ and a power-law slope ≳1.25. We also use this result to constrain the initial mass function in the Galactic center by considering different star formation scenarios.
High-resolution soft x-ray photoionization studies of selected molecules
International Nuclear Information System (INIS)
Hudson, E.A.
1993-08-01
Near-edge soft x-ray photoionization spectra were measured for CO, SF 6 , H 2 S, and D 2 S in the gas phase, using the Free University of Berlin plane-grating SX-700-II monochromator at the synchrotron radiation source BESSY. Photoionization spectra of carbon monoxide were measured near the carbon and oxygen K edges. Vibrational spacings and bond lengths are derived for several resonances. Results are consistent with equivalent-core model and indicate the different influences of the carbon and oxygen Is core holes. Corresponding spectra of H 2 CO and D 2 CO were also measured. Assignment of complex vibrational structure in valence-shell and Rydberg resonances is facilitated by comparison of spectra for the two isotopic species. Geometric and vibrational parameters are derived for several carbon 1s core-excited states. Isotopic shifts are observed in the energies and linewidths of some core-excited states. Sulfur hexafluoride photoionization spectra, measured near the sulfur L 2,3 edges, show several series of weak, narrow Rydberg resonances. High resolution and good counting statistics allow a complete assignment of these states. Lineshapes of the broad inner-well resonances are analyzed to establish the magnitudes of vibrational and lifetime broadening in these states. Spectra of the H 2 S and D 2 S molecules were also measured near the sulfur L 2,3 edges. Besides lower-energy transitions to inner-well states, a complex manifold of overlapping Rydberg resonances is observed. The rich fine structure of these states arises mainly from removal of orbital degeneracies in molecular field. Additional structure due to vibrational excitations in the final state is identified by comparison of the spectra for the two isotopic species
Calculation of the characteristics of carbon dioxide TEA photoionization lasers
Energy Technology Data Exchange (ETDEWEB)
Aver' yanov, N E; Baloshin, Yu A; Gerke, M N; Dernyatin, A I; Khurgin, Ya B
1979-01-01
A mathematical model is proposed for studying the characteristics of a carbon dioxide photoionization laser with pressures of the active mixture of the order of one atmosphere. The kinetics of the CO/sub 2/ molecules is described in terms of population of the group of lower vibrational levels. The part played by N/sub 2/ molecules in the general system of kinetic equations is accounted for by a harmonic oscillator model with Boltzmann population of vibrational levels and the corresponding vibrational temperature. A diagram is given of the fundamental kinetic processes in the proposed model for a TEA laser. The results of calculations are compared with a previously proposed model and with experimental data for a carbon dioxide TEA photoionization laser using preionization by ultraviolet radiation and operating in the semi-selfmaintained discharge mode. The active mixture was CO/sub 2/:N/sub 2/:He=1:1:8. It was found that optimum mixtures for maximum power are those with ratios of CO/sub 2/:N/sub 2/He=5:45:50, 10:40:50 and 5:55:40. The helium molecules supply most of the photoelectrons, and the additives give a uv spectrum that is optimum for photoionization of He. The CO/sub 2/ is the lasing molecule, but absorbs uv radiation, and therefore the optimum CO/sub 2/ concentration is low. The influence that dissociation of CO/sub 2/ molecules has on the laser depends on the electron concentration in the main discharge. Any model that reliably describes laser characteristics must take account of dissociation of the lasing molecules by means of some factor that shows how many molecules are dissociated by uv radiation, although the dissociation by electron impact can be disregarded.
Theoretical and expert system approach to photoionization theories
Directory of Open Access Journals (Sweden)
Petrović Ivan D.
2016-01-01
Full Text Available The influence of the ponderomotive and the Stark shifts on the tunneling transition rate was observed, for non-relativistic linearly polarized laser field for alkali atoms, with three different theoretical models, the Keldysh theory, the Perelomov, Popov, Terent'ev (PPT theory, and the Ammosov, Delone, Krainov (ADK theory. We showed that aforementioned shifts affect the transition rate differently for different approaches. Finally, we presented a simple expert system for analysis of photoionization theories.
Exploring the dust content of galactic winds with Herschel - II. Nearby dwarf galaxies
McCormick, Alexander; Veilleux, Sylvain; Meléndez, Marcio; Martin, Crystal L.; Bland-Hawthorn, Joss; Cecil, Gerald; Heitsch, Fabian; Müller, Thomas; Rupke, David S. N.; Engelbracht, Chad
2018-06-01
We present the results from an analysis of deep Herschel Space Observatory observations of six nearby dwarf galaxies known to host galactic-scale winds. The superior far-infrared sensitivity and angular resolution of Herschel have allowed detection of cold circumgalactic dust features beyond the stellar components of the host galaxies traced by Spitzer 4.5 μm images. Comparisons of these cold dust features with ancillary data reveal an imperfect spatial correlation with the ionized gas and warm dust wind components. We find that typically ˜10-20 per cent of the total dust mass in these galaxies resides outside of their stellar discs, but this fraction reaches ˜60 per cent in the case of NGC 1569. This galaxy also has the largest metallicity (O/H) deficit in our sample for its stellar mass. Overall, the small number of objects in our sample precludes drawing strong conclusions on the origin of the circumgalactic dust. We detect no statistically significant trends with star formation properties of the host galaxies, as might be expected if the dust were lifted above the disc by energy inputs from ongoing star formation activity. Although a case for dust entrained in a galactic wind is seen in NGC 1569, in all cases, we cannot rule out the possibility that some of the circumgalactic dust might be associated instead with gas accreted or removed from the disc by recent galaxy interaction events, or that it is part of the outer gas-rich portion of the disc that lies below the sensitivity limit of the Spitzer 4.5 μm data.
Principles of Stellar Interferometry
Glindemann, Andreas
2011-01-01
Over the last decade, stellar interferometry has developed from a specialist tool to a mainstream observing technique, attracting scientists whose research benefits from milliarcsecond angular resolution. Stellar interferometry has become part of the astronomer’s toolbox, complementing single-telescope observations by providing unique capabilities that will advance astronomical research. This carefully written book is intended to provide a solid understanding of the principles of stellar interferometry to students starting an astronomical research project in this field or to develop instruments and to astronomers using interferometry but who are not interferometrists per se. Illustrated by excellent drawings and calculated graphs the imaging process in stellar interferometers is explained starting from first principles on light propagation and diffraction wave propagation through turbulence is described in detail using Kolmogorov statistics the impact of turbulence on the imaging process is discussed both f...
EG Andromedae: A New Orbit and Additional Evidence for a Photoionized Wind
Kenyon, Scott J.; Garcia, Michael R.
2016-07-01
We analyze a roughly 20 yr set of spectroscopic observations for the symbiotic binary EG And. Radial velocities derived from echelle spectra are best fit with a circular orbit having an orbital period of P = 483.3 ± 1.6 days and semi-amplitude K = 7.34 ± 0.07 km s-1. Combined with previous data, these observations rule out an elliptical orbit at the 10σ level. Equivalent widths of H I Balmer emission lines and various absorption features vary in phase with the orbital period. Relative to the radius of the red giant primary, the apparent size of the H II region is consistent with a model where a hot secondary star with effective temperature T h ≈ 75,000 K ionizes the wind from the red giant.
Advanced stellarator power plants
International Nuclear Information System (INIS)
Miller, R.L.
1994-01-01
The stellarator is a class of helical/toroidal magnetic fusion devices. Recent international progress in stellarator power plant conceptual design is reviewed and comparisons in the areas of physics, engineering, and economics are made with recent tokamak design studies
Probing photo-ionization: experiments on positive streamers in pure gases and mixtures
International Nuclear Information System (INIS)
Nijdam, S; Van de Wetering, F M J H; Blanc, R; Van Veldhuizen, E M; Ebert, U
2010-01-01
Positive streamers are thought to propagate by photo-ionization; the parameters of photo-ionization depend on the nitrogen : oxygen ratio. Therefore we study streamers in nitrogen with 20%, 0.2% and 0.01% oxygen and in pure nitrogen as well as in pure oxygen and argon. Our new experimental set-up guarantees contamination of the pure gases to be well below 1 ppm. Streamers in oxygen are difficult to measure as they emit considerably less light in the sensitivity range of our fast ICCD camera than the other gases. Streamers in pure nitrogen and in all nitrogen-oxygen mixtures look generally similar, but become somewhat thinner and branch more with decreasing oxygen content. In pure nitrogen the streamers can branch so much that they resemble feathers. This feature is even more pronounced in pure argon, with approximately 10 2 hair tips cm -3 in the feathers at 200 mbar; this density can be interpreted as the free electron density creating avalanches towards the streamer stem. It is remarkable that the streamer velocity is essentially the same for similar voltage and pressure in all nitrogen-oxygen mixtures as well as in pure nitrogen, while the oxygen concentration and therefore the photo-ionization lengths vary by more than five orders of magnitude. Streamers in argon have essentially the same velocity as well. The physical similarity of streamers at different pressures is confirmed in all gases; the minimal diameters are smaller than in earlier measurements.
Probing photo-ionization: experiments on positive streamers in pure gases and mixtures
Energy Technology Data Exchange (ETDEWEB)
Nijdam, S; Van de Wetering, F M J H; Blanc, R; Van Veldhuizen, E M; Ebert, U, E-mail: s.nijdam@tue.n [Eindhoven University of Technology, Department Applied Physics, PO Box 513, 5600 MB Eindhoven (Netherlands)
2010-04-14
Positive streamers are thought to propagate by photo-ionization; the parameters of photo-ionization depend on the nitrogen : oxygen ratio. Therefore we study streamers in nitrogen with 20%, 0.2% and 0.01% oxygen and in pure nitrogen as well as in pure oxygen and argon. Our new experimental set-up guarantees contamination of the pure gases to be well below 1 ppm. Streamers in oxygen are difficult to measure as they emit considerably less light in the sensitivity range of our fast ICCD camera than the other gases. Streamers in pure nitrogen and in all nitrogen-oxygen mixtures look generally similar, but become somewhat thinner and branch more with decreasing oxygen content. In pure nitrogen the streamers can branch so much that they resemble feathers. This feature is even more pronounced in pure argon, with approximately 10{sup 2} hair tips cm{sup -3} in the feathers at 200 mbar; this density can be interpreted as the free electron density creating avalanches towards the streamer stem. It is remarkable that the streamer velocity is essentially the same for similar voltage and pressure in all nitrogen-oxygen mixtures as well as in pure nitrogen, while the oxygen concentration and therefore the photo-ionization lengths vary by more than five orders of magnitude. Streamers in argon have essentially the same velocity as well. The physical similarity of streamers at different pressures is confirmed in all gases; the minimal diameters are smaller than in earlier measurements.
International Nuclear Information System (INIS)
Lim, Gwon; Jeong, Do Young; Ko, Kwang Hoon; Kim, Jae Woo; Kim, Taek Soo; Rho, Sipyo; Kim, Cheol Jung
2003-01-01
We have constructed the frequency-locked pulsed dye laser system. It is composed with a GIM-type oscillator and 3 stage longitudinally pumped amplifiers. The pump laser is the second harmonic of pulse Nd:YAG laser at the repetition rate of 6 kHz. Frequency-locking of dye laser oscillator is actively controlled by the feedback loop between a photoionization signal of T1-203 isotope and a wavelength tuning control. The tuning mirror rotates the order of micro degree per a step of step motor. Feedback system for frequency locking is operated with a PC-based control interface, including the data analysis of photoionization signals and the wavelength control using step pumping method for a medical application. Therefor, the dye laser has to be locked at 583.66 nm for SHG or BBO crystal. With the frequency-locking system, the photoionization experiment has been done for more than 10 hours.
Anatomy of the AGN in NGC 5548. IX. Photoionized emission features in the soft X-ray spectra
Mao, Junjie; Kaastra, J. S.; Mehdipour, M.; Gu, Liyi; Costantini, E.; Kriss, G. A.; Bianchi, S.; Branduardi-Raymont, G.; Behar, E.; Di Gesu, L.; Ponti, G.; Petrucci, P.-O.; Ebrero, J.
2018-04-01
The X-ray narrow emission line region (NELR) of the archetypal Seyfert 1 galaxy NGC 5548 has been interpreted as a single-phase photoionized plasma that is absorbed by some of the warm absorber components. This scenario requires those overlaying warm absorber components to have larger distance (to the central engine) than the X-ray NELR, which is not fully consistent with the distance estimates found in the literature. Therefore, we reanalyze the high-resolution spectra obtained in 2013-2014 with the Reflection Grating Spectrometer (RGS) aboard XMM-Newton to provide an alternative interpretation of the X-ray narrow emission features. We find that the X-ray narrow emission features in NGC 5548 can be described by a two-phase photoionized plasma with different ionization parameters (logξ = 1.3 and 0.1) and kinematics (vout = -50 and -400 km s-1), and no further absorption by the warm absorber components. The X-ray and optical NELR might be the same multi-phase photoionized plasma. Both X-ray and optical NELR have comparable distances, asymmetric line profiles, and the underlying photoionized plasma is turbulent and compact in size. The X-ray NELR is not the counterpart of the UV/X-ray absorber outside the line of sight because their distances and kinematics are not consistent. In addition, X-ray broad emission features that we find in the spectrum can be accounted for by a third photoionized emission component. The RGS spectrum obtained in 2016 is analyzed as well, where the luminosity of most prominent emission lines (the O VII forbidden line and O VIII Lyα line) are the same (at a 1σ confidence level) as in 2013-2014.
Use of the stellarator expansion to investigate plasma equilibrium in modular stellarators
International Nuclear Information System (INIS)
Anania, G.; Johnson, J.L.; Weimer, K.E.
1982-11-01
A numerical code utilizing a large-aspect ratio, small-helical-distortion expansion is developed and used to investigate the effect of plasma currents on stellarator equilibrium. Application to modular stellarator configurations shows that a large rotational transform, and hence large coil deformation, is needed to achieve high-beta equilibria
Photoionization in the Precursor of Laser Supported Detonation by Ultraviolet Radiation
International Nuclear Information System (INIS)
Shimamura, Kohei; Michigami, Keisuke; Wang, Bin; Komurasaki, Kimiya; Arakawa, Yoshihiro
2011-01-01
The propagation mechanism of laser-supported detonation (LSD) is important for designing laser propulsion for a detonation type thruster. The purpose of this work to was to confirm that photo-ionization in precursor is the predominant LSD sustainment mechanism. First of all, we tried to investigate the dependency of LSD duration on ambient gas species, air and argon. We took a series of high-speed images using the laser shadow-graphy. Besides, to estimate the UV photons emitted from the plasma, we used plasma emission spectroscopy and determined the electron temperature and density. As a result, the LSD duration of argon plasma and air plasma are 0.7 μs and 0.3 μs, resp. Besides, argon plasma emitted 10 10 to 10 14 photons/seconds, which was higher than air plasma. These results reveal that LSD propagation depends on the photon-contributing photoionization. The threshold photon-emission rate of LSD termination gives the elucidation of the LSD termination condition.
The Monte Carlo photoionization and moving-mesh radiation hydrodynamics code CMACIONIZE
Vandenbroucke, B.; Wood, K.
2018-04-01
We present the public Monte Carlo photoionization and moving-mesh radiation hydrodynamics code CMACIONIZE, which can be used to simulate the self-consistent evolution of HII regions surrounding young O and B stars, or other sources of ionizing radiation. The code combines a Monte Carlo photoionization algorithm that uses a complex mix of hydrogen, helium and several coolants in order to self-consistently solve for the ionization and temperature balance at any given type, with a standard first order hydrodynamics scheme. The code can be run as a post-processing tool to get the line emission from an existing simulation snapshot, but can also be used to run full radiation hydrodynamical simulations. Both the radiation transfer and the hydrodynamics are implemented in a general way that is independent of the grid structure that is used to discretize the system, allowing it to be run both as a standard fixed grid code, but also as a moving-mesh code.
International Nuclear Information System (INIS)
Kivimaeki, A.; Alvarez-Ruiz, J.; Coreno, M.; Simone, M. de; Moise, A.; Partanen, L.; Richter, R.; Stankiewicz, M.
2010-01-01
Low-energy photoelectron-vacuum ultraviolet (VUV) photon coincidences have been measured using synchrotron radiation excitation in the inner-valence region of the nitric oxide molecule. The capabilities of the coincidence set-up were demonstrated by detecting the 2s -1 → 2p -1 radiative transitions in coincidence with the 2s photoelectron emission in Ne. In NO, the observed coincidence events are attributed to dissociative photoionization with excitation, whereby photoelectron emission is followed by fragmentation of excited NO + ions into O + + N* or N + + O* and VUV emission from an excited neutral fragment. The highest coincidence rate occurs with the opening of ionization channels which are due to correlation satellites of the 3σ photoionization. The decay time of VUV photon emission was also measured, implying that specific excited states of N atoms contribute significantly to observed VUV emission.
Stellar CME candidates: towards a stellar CME-flare relation
Paraskevi Moschou, Sofia; Drake, Jeremy J.; Cohen, Ofer; Alvarado-Gomez, Julian D.; Garraffo, Cecilia
2018-06-01
For decades the Sun has been the only star that allowed for direct CME observations. Recently, with the discovery of multiple extrasolar systems, it has become imperative that the role of stellar CMEs be assessed in the context of exoplanetary habitability. Solar CMEs and flares show a higher association with increasing flaring energy, with strong flares corresponding to large and fast CMEs. As argued in earlier studies, extrasolar environments around active stars are potentially dominated by CMEs, as a result of their extreme flaring activity. This has strong implications for the energy budget of the system and the atmospheric erosion of orbiting planets.Nevertheless, with current instrumentation we are unable to directly observe CMEs in even the closest stars, and thus we have to look for indirect techniques and observational evidence and signatures for the eruption of stellar CMEs. There are three major observational techniques for tracing CME signatures in other stellar systems, namely measuring Type II radio bursts, Doppler shifts in UV/optical lines or transient absorption in the X-ray spectrum. We present observations of the most probable stellar CME candidates captured so far and examine the different observational techniques used together with their levels of uncertainty. Assuming that they were CMEs, we try to asses their kinematic and energetic characteristics and place them in an extension of the well-established solar CME-flare energy scaling law. We finish by discussing future observations for direct measurements.
Absolute measurements of chlorine Cl+ cation single photoionization cross section
Hernandez, E. M.; Juarez, A. M.; Kilcoyne, A. L. D.; Aguilar, A.; Hernandez, L.; Antillon, A.; Macaluso, D.; Morales-Mori, A.; Gonzalez-Magana, O.; Hanstorp, D.; Covington, A. M.; Davis, V.; Calabrese, D.; Hinojosa, G.
The photoionization of Cl+ leading to Cl2+ was measured in the photon energy range of 19.5-28.0 eV. A spectrum with a photon energy resolution of 15 meV normalized to absolute cross-section measurements is presented. The measurements were carried out by merging a Cl+ ion beam with a photon beam of
Stellarator fusion neutronics research in Australia
International Nuclear Information System (INIS)
Zimin, S.; Cross, R.C.
1997-01-01
The new status of the H-INF Heliac Stellaralor as a National Facility and the signed international Implementing Agreement on 'Collaboration in the Development of the Stellarator Concept' represents a significant encouragement for further fusion research in Australia. In this report the future of fusion research in Australia is discussed with special attention being paid to the importance of Stellarator power plant studies and in particular stellarator fusion neutronics. The main differences between tokamak and stellarator neutronics analyses are identified, namely the neutron wall loading, geometrical modelling and total heating in in-vessel reactor components including toroidal field (TF) coils. Due to the more complicated nature of stellarator neutronics analyses, simplified approaches to fusion neutronics already developed for tokamaks are expected to be even more important and widely used for designing a Conceptual Stellarator Power Plant
2D hydrodynamic simulations of super star cluster winds in a bimodal regime
Czech Academy of Sciences Publication Activity Database
Wünsch, Richard; Palouš, Jan; Tenorio-Tagle, G.; Silich, S.
2009-01-01
Roč. 324, 2-4 (2009), s. 219-223 ISSN 0004-640X R&D Projects: GA MŠk(CZ) LC06014 Institutional research plan: CEZ:AV0Z10030501 Keywords : stellar winds * star clusters * dynamics of ISM Subject RIV: BN - Astronomy, Celestial Mechanics, Astrophysics Impact factor: 1.404, year: 2009
Photoionization sensor CES for non-invasive medical diagnostics
Mustafaev, Aleksandr; Rastvorova, Iuliia; Khobnya, Kristina; Podenko, Sofia
2016-10-01
Method CES (collisional electron spectroscopy), patented in Russia, the USA, Japan, China, Germany and Britain, allows to analyze the gaseous mixtures using electron spectroscopy under high pressures up to atmospheric without using vacuum. The design of VUV photoionization detector was developed based on this method. Such detector is used as a portable gas analyzer for continuous personal bio-medical monitoring. This detector measures energy of electrons produced in ionization with resonance photons, whose wavelength situated in the vacuum ultraviolet (VUV). Nowadays, micro plasma source of such photons on resonant line of Kr with energy of 10,6 eV is developed. Only impurities are ionized and detected by the VUV-emission, meanwhile the main components of air stay neutral that reduces background signal and increases the sensibility along with accuracy. The experimental facilities with VUV photoionization sensors CES are constructed with the overall sizes about 10*10*1 mm. The watt consumption may comprise less than 1W. Increase of electrometer amplifier's sensibility and more high-aperture construction are used today to increase the sensibility of CES-detectors. The wide range of detectable molecules and high sensitivity allow the development of portable device, which can become the base of the future preventive medicine. Work supported by Foundation for Assistance to Small Innovative Enterprises in Science and Technology.
Attosecond delays in photoionization: time and quantum mechanics
International Nuclear Information System (INIS)
Maquet, Alfred; Caillat, Jérémie; Taïeb, Richard
2014-01-01
This article addresses topics regarding time measurements performed on quantum systems. The motivation is linked to the advent of ‘attophysics’ which makes feasible to follow the motion of electrons in atoms and molecules, with time resolution at the attosecond (1 as = 10 −18 s) level, i.e. at the natural scale for electronic processes in these systems. In this context, attosecond ‘time-delays’ have been recently measured in experiments on photoionization and the question arises if such advances could cast a new light on the still active discussion on the status of the time variable in quantum mechanics. One issue still debatable is how to decide whether one can define a quantum time operator with eigenvalues associated to measurable ‘time-delays’, or time is a parameter, as it is implicit in the Newtonian classical mechanics. One objective of this paper is to investigate if the recent attophysics-based measurements could shed light on this parameter–operator conundrum. To this end, we present here the main features of the theory background, followed by an analysis of the experimental schemes that have been used to evidence attosecond ‘time-delays’ in photoionization. Our conclusion is that these results reinforce the view that time is a parameter which cannot be defined without reference to classical mechanics. (tutorial)
Attosecond time delays in the photoionization of noble gas atoms studied in TDLDA
International Nuclear Information System (INIS)
Magrakvelidze, Maia; Chakraborty, Himadri; Madjet, Mohamed
2015-01-01
We perform time-dependent local density functional calculations of the quantum phase and time delays of valence photoionization of noble gas atoms. Results may be accessed by XUV-IR interferometric metrology. (paper)
Inner-shell photoionization and core-hole decay of Xe and XeF2.
Southworth, Stephen H; Wehlitz, Ralf; Picón, Antonio; Lehmann, C Stefan; Cheng, Lan; Stanton, John F
2015-06-14
Photoionization cross sections and partial ion yields of Xe and XeF2 from Xe 3d(5/2), Xe 3d(3/2), and F 1s subshells in the 660-740 eV range are compared to explore effects of the F ligands. The Xe 3d-ϵf continuum shape resonances dominate the photoionization cross sections of both the atom and molecule, but prominent resonances appear in the XeF2 cross section due to nominal excitation of Xe 3d and F 1s electrons to the lowest unoccupied molecular orbital (LUMO), a delocalized anti-bonding MO. Comparisons of the ion products from the atom and molecule following Xe 3d photoionization show that the charge-state distribution of Xe ions is shifted to lower charge states in the molecule along with production of energetic F(+) and F(2+) ions. This suggests that, in decay of a Xe 3d core hole, charge is redistributed to the F ligands and the system dissociates due to Coulomb repulsion. The ion products from excitation of the F 1s-LUMO resonance are different and show strong increases in the yields of Xe(+) and F(+) ions. The subshell ionization thresholds, the LUMO resonance energies, and their oscillator strengths are calculated by relativistic coupled-cluster methods and agree well with measurements.
International Nuclear Information System (INIS)
Feltzing, S; Bensby, T
2008-01-01
The study of the Milky Way stellar discs in the context of galaxy formation is discussed. In particular, we explore the properties of the Milky Way disc using a new sample of about 550 dwarf stars for which we have recently obtained elemental abundances and ages based on high-resolution spectroscopy. For all the stars we also have full kinematic information as well as information about their stellar orbits. We confirm results from previous studies that the thin and the thick discs have distinct abundance patterns. But we also explore a larger range of orbital parameters than what has been possible in our previous studies. Several new results are presented. We find that stars that reach high above the Galactic plane and have eccentric orbits show remarkably tight abundance trends. This implies that these stars formed out of well-mixed gas that had been homogenized over large volumes. We find some evidence that suggest that the event that most likely caused the heating of this stellar population happened a few billion years ago. Through a simple, kinematic exploration of stars with super-solar [Fe/H], we show that the solar neighbourhood contains metal-rich, high velocity stars that are very likely associated with the thick disc. Additionally, the HR1614 moving group and the Hercules and Arcturus stellar streams are discussed and it is concluded that, probably, a large fraction of the groups and streams so far identified in the disc are the result of evolution and interactions within the stellar disc rather than being dissolved stellar clusters or engulfed dwarf galaxies.
THE TRANSITION MASS-LOSS RATE: CALIBRATING THE ROLE OF LINE-DRIVEN WINDS IN MASSIVE STAR EVOLUTION
Energy Technology Data Exchange (ETDEWEB)
Vink, Jorick S.; Graefener, Goetz, E-mail: jsv@arm.ac.uk [Armagh Observatory, College Hill, BT61 9DG Armagh (United Kingdom)
2012-06-01
A debate has arisen regarding the importance of stationary versus eruptive mass loss for massive star evolution. The reason is that stellar winds have been found to be clumped, which results in the reduction of unclumped empirical mass-loss rates. Most stellar evolution models employ theoretical mass-loss rates which are already reduced by a moderate factor of {approx_equal}2-3 compared to non-corrected empirical rates. A key question is whether these reduced rates are of the correct order of magnitude, or if they should be reduced even further, which would mean that the alternative of eruptive mass loss becomes necessary. Here we introduce the transition mass-loss rate M-dot{sub trans} between O and Wolf-Rayet stars. Its novelty is that it is model independent. All that is required is postulating the spectroscopic transition point in a given data set, and determining the stellar luminosity, which is far less model dependent than the mass-loss rate. The transition mass-loss rate is subsequently used to calibrate stellar wind strength by its application to the Of/WNh stars in the Arches cluster. Good agreement is found with two alternative modeling/theoretical results, suggesting that the rates provided by current theoretical models are of the right order of magnitude in the {approx}50 M{sub Sun} mass range. Our results do not confirm the specific need for eruptive mass loss as luminous blue variables, and current stellar evolution modeling for Galactic massive stars seems sound. Mass loss through alternative mechanisms might still become necessary at lower masses, and/or metallicities, and the quantification of alternative mass loss is desirable.
THE TRANSITION MASS-LOSS RATE: CALIBRATING THE ROLE OF LINE-DRIVEN WINDS IN MASSIVE STAR EVOLUTION
International Nuclear Information System (INIS)
Vink, Jorick S.; Gräfener, Götz
2012-01-01
A debate has arisen regarding the importance of stationary versus eruptive mass loss for massive star evolution. The reason is that stellar winds have been found to be clumped, which results in the reduction of unclumped empirical mass-loss rates. Most stellar evolution models employ theoretical mass-loss rates which are already reduced by a moderate factor of ≅2-3 compared to non-corrected empirical rates. A key question is whether these reduced rates are of the correct order of magnitude, or if they should be reduced even further, which would mean that the alternative of eruptive mass loss becomes necessary. Here we introduce the transition mass-loss rate M-dot trans between O and Wolf-Rayet stars. Its novelty is that it is model independent. All that is required is postulating the spectroscopic transition point in a given data set, and determining the stellar luminosity, which is far less model dependent than the mass-loss rate. The transition mass-loss rate is subsequently used to calibrate stellar wind strength by its application to the Of/WNh stars in the Arches cluster. Good agreement is found with two alternative modeling/theoretical results, suggesting that the rates provided by current theoretical models are of the right order of magnitude in the ∼50 M ☉ mass range. Our results do not confirm the specific need for eruptive mass loss as luminous blue variables, and current stellar evolution modeling for Galactic massive stars seems sound. Mass loss through alternative mechanisms might still become necessary at lower masses, and/or metallicities, and the quantification of alternative mass loss is desirable.
Injection and laser acceleration of ions based on the resonant surface photoionization
International Nuclear Information System (INIS)
Antsiferov, V.V.; Smirnov, G.I.; Telegin, G.G.
1993-01-01
The collective effects have been investigated of the injection and acceleration of the ion beams due to the resonant surface photoionization. The considered scheme of the laser accelerator allows to obtain positive ions with relativistic velocities. 11 refs., 2 figs
Sterling, N. C.; Witthoeft, Michael
2011-01-01
We present multi-configuration Breit-Pauli AUTOSTRUCTURE calculations of distorted-wave photoionization (PI) cross sections. and total and partial final-state resolved radiative recombination (RR) and dielectronic recombination (DR) rate coefficients for the first six ions of the trans-iron element Se. These calculations were motivated by the recent detection of Se emission lines in a large number of planetary nebulae. Se is a potentially useful tracer of neutron-capture nucleosynthesis. but accurate determinations of its abundance in photoionized nebulae have been hindered by the lack of atomic data governing its ionization balance. Our calculations were carried out in intermediate coupling with semi re1ativistic radial wavefunctions. PI and recombination data were determined for levels within the ground configuration of each ion, and experimental PI cross-section measurements were used to benchmark our results. For DR, we allowed (Delta)n = 0 core excitations, which are important at photoionized plasma temperatures. We find that DR is the dominant recombination process for each of these Se ions at temperatures representative of photoionized nebulae (approx.10(exp 4) K). In order to estimate the uncertainties of these data, we compared results from three different configuration-interaction expansions for each ion, and also tested the sensitivity of the results to the radial scaling factors in the structure calculations. We find that the internal uncertainties are typically 30-50% for the direct PI cross sections and approx.10% for the computed RR rate coefficients, while those for low-temperature DR can be considerably larger (from 15-30% up to two orders of magnitude) due to the unknown energies of near-threshold autoionization resonances. These data are available at the CDS, and fitting coefficients to the total RR and DR rate coefficients are presented. The results are suitable for incorporation into photoionization codes used to numerically simulate
EG ANDROMEDAE: A NEW ORBIT AND ADDITIONAL EVIDENCE FOR A PHOTOIONIZED WIND
International Nuclear Information System (INIS)
Kenyon, Scott J.; Garcia, Michael R.
2016-01-01
We analyze a roughly 20 yr set of spectroscopic observations for the symbiotic binary EG And. Radial velocities derived from echelle spectra are best fit with a circular orbit having an orbital period of P = 483.3 ± 1.6 days and semi-amplitude K = 7.34 ± 0.07 km s −1 . Combined with previous data, these observations rule out an elliptical orbit at the 10 σ level. Equivalent widths of H i Balmer emission lines and various absorption features vary in phase with the orbital period. Relative to the radius of the red giant primary, the apparent size of the H ii region is consistent with a model where a hot secondary star with effective temperature T h ≈ 75,000 K ionizes the wind from the red giant.
EG ANDROMEDAE: A NEW ORBIT AND ADDITIONAL EVIDENCE FOR A PHOTOIONIZED WIND
Energy Technology Data Exchange (ETDEWEB)
Kenyon, Scott J. [Smithsonian Astrophysical Observatory, 60 Garden Street, Cambridge, MA 02138 (United States); Garcia, Michael R., E-mail: skenyon@cfa.harvard.edu, E-mail: michael.r.garcia@nasa.gov [NASA Headquarters, Mail Suite 3Y28, 300 E Street SW, Washington, DC 20546-0001 (United States)
2016-07-01
We analyze a roughly 20 yr set of spectroscopic observations for the symbiotic binary EG And. Radial velocities derived from echelle spectra are best fit with a circular orbit having an orbital period of P = 483.3 ± 1.6 days and semi-amplitude K = 7.34 ± 0.07 km s{sup −1}. Combined with previous data, these observations rule out an elliptical orbit at the 10 σ level. Equivalent widths of H i Balmer emission lines and various absorption features vary in phase with the orbital period. Relative to the radius of the red giant primary, the apparent size of the H ii region is consistent with a model where a hot secondary star with effective temperature T{sub h} ≈ 75,000 K ionizes the wind from the red giant.
Stellar origin of the 22Ne excess in cosmic rays
International Nuclear Information System (INIS)
Casse, M.; Paul, J.A.
1982-01-01
The 22 Ne excess at the cosmic-ray source is discussed in terms of a 22 Ne-rich component injected and accelerated by carbon-rich Wolf-Rayet stars. The overabundance of 22 Ne relative to 20 Ne predicted at the surface of these stars is estimated to a factor approx.120 with respect to solar system abundances. In order to give rise to a 22 Ne excess of about 3 at the cosmic-ray sources as inferred from observations, the carbon-rich Wolf-Rayet contribution to the primary cosmic-ray flux is to be at maximum 1/60. This component would be energized by strong stellar winds producing quasi-standing shocks around the Wolf-Rayet stars
Energy Technology Data Exchange (ETDEWEB)
Agertz, Oscar; Kravtsov, Andrey V.; Leitner, Samuel N.; Gnedin, Nickolay Y.
2013-05-21
We investigate the momentum and energy budget of stellar feedback during different stages of stellar evolution, and study its impact on the interstellar medium (ISM) using simulations of local star-forming regions and galactic disks at the resolution affordable in modern cosmological zoom-in simulations. In particular, we present a novel subgrid model for the momentum injection due to radiation pressure and stellar winds from massive stars during early, pre-supernova (pre-SN) evolutionary stages of young star clusters. Early injection of momentum acts to clear out dense gas in star-forming regions, hence limiting star formation. The reduced gas density mitigates radiative losses of thermal feedback energy from subsequent SN explosions. The detailed impact of stellar feedback depends sensitively on the implementation and choice of parameters. Somewhat encouragingly, we find that implementations in which feedback is efficient lead to approximate self-regulation of the global star formation efficiency. We compare simulation results using our feedback implementation to other phenomenological feedback methods, where thermal feedback energy is allowed to dissipate over timescales longer than the formal gas cooling time. We find that simulations with maximal momentum injection suppress star formation to a similar degree as is found in simulations adopting adiabatic thermal feedback. However, different feedback schemes are found to produce significant differences in the density and thermodynamic structure of the ISM, and are hence expected to have a qualitatively different impact on galaxy evolution.