A quantum cascade phonon-polariton laser
Ohtani, Keita; Bosco, Lorenzo; Beck, Mattias; Faist, Jérôme
2016-01-01
We report a laser that coherently emits phonon-polaritons, quasi-particles arising from the coupling between photons and transverse optical phonons. The gain is provided by an intersubband transition in a quantum cascade structure. The polaritons at h$\
2005-05-09
Carbon Nanotubes with Enhanced K(T) CNT in CNT Yarns and Oriented CNT bucky- aerogels 4Anvar A. Zakhidov, University of Texas at Dallas Our Main...CNT Fibers and Yarns and - Oriented CNT-ribbon aerogels 50Anvar A. Zakhidov, University of Texas at Dallas PHONON TRANSISTOR in NANOTUBE FIBERS with...100µm) of copper and gold are much lower: Dcopper = 117 mm2/s, Dgold = 130 mm2/s. 60Anvar A. Zakhidov, University of Texas at Dallas Multifunctional
Electron-phonon equilibration in laser-heated gold films
White, T. G.; Mabey, P.; Gericke, D. O.; Hartley, N. J.; Doyle, H. W.; McGonegle, D.; Rackstraw, D. S.; Higginbotham, A.; Gregori, G.
2014-07-01
By irradiating a thin metal foil with an intense short-pulse laser, we have created a uniform system far from equilibrium. The deposited energy is initially deposited only within the electronic subsystem, and the subsequent evolution of the system is determined by the details of the electron-phonon coupling. Here, we measure the time evolution of the lattice parameter through multilayer Bragg diffraction and compare the result to classical molecular dynamic simulations to determine the lattice temperature. The electron-ion coupling constant for gold is then determined by comparison with the evolution of a two-temperature electron-phonon system.
Electron and phonon dynamics in laser short pulses-heated metals
Pietanza, L. D.; Colonna, G.; Capitelli, M.
2005-07-01
The simultaneous electron and phonon relaxation dynamic in a metal film subjected to a laser pulse has been theoretically investigated. A system of two coupled time- and energy-dependent Boltzmann equations describing the electron and phonon dynamics has been numerically solved. The collision processes considered are electron-electron (e-e) and electron-phonon (e-p) collisions. Our results show the non-equilibrium electron distribution and the electron and phonon relaxation dynamics both after a femtosecond and a picosecond laser perturbations.
Laser structuring for control of coupling between THz light and phonon modes
Wang, X W; Balcytis, A; Kasalynas, I; Jakstas, V; Janonis, V; Venckevicius, R; Buividas, R; Appadoo, D; Valusis, G; Juodkazis, S
2016-01-01
Modification of surface and volume of sapphire is shown to affect reflected and transmitted light at THz spectral range. Structural modifications were made using ultra-short 230 fs laser pulses at 1030 nm and 257.5 nm wavelengths forming surface ripples of ~250 nm and 60 nm period, respectively. Softening of the transverse optical phonon TO1 mode due to disorder was the most pronounced in reflection from laser ablated surface. It is shown that sub-surface periodic patterns of laser damage sites have also modified reflection spectrum due to coupling of THz radiation with phonons. Application potential of laser structuring and disordering for phononic engineering is discussed.
Energy Technology Data Exchange (ETDEWEB)
Giri, Ashutosh; Hopkins, Patrick E., E-mail: phopkins@virginia.edu [Department of Mechanical and Aerospace Engineering, University of Virginia, Charlottesville, Virginia 22904 (United States)
2015-12-07
Several dynamic thermal and nonthermal scattering processes affect ultrafast heat transfer in metals after short-pulsed laser heating. Even with decades of measurements of electron-phonon relaxation, the role of thermal vs. nonthermal electron and phonon scattering on overall electron energy transfer to the phonons remains unclear. In this work, we derive an analytical expression for the electron-phonon coupling factor in a metal that includes contributions from equilibrium and nonequilibrium distributions of electrons. While the contribution from the nonthermal electrons to electron-phonon coupling is non-negligible, the increase in the electron relaxation rates with increasing laser fluence measured by thermoreflectance techniques cannot be accounted for by only considering electron-phonon relaxations. We conclude that electron-electron scattering along with electron-phonon scattering have to be considered simultaneously to correctly predict the transient nature of electron relaxation during and after short-pulsed heating of metals at elevated electron temperatures. Furthermore, for high electron temperature perturbations achieved at high absorbed laser fluences, we show good agreement between our model, which accounts for d-band excitations, and previous experimental data. Our model can be extended to other free electron metals with the knowledge of the density of states of electrons in the metals and considering electronic excitations from non-Fermi surface states.
Giri, Ashutosh; Hopkins, Patrick E.
2015-12-01
Several dynamic thermal and nonthermal scattering processes affect ultrafast heat transfer in metals after short-pulsed laser heating. Even with decades of measurements of electron-phonon relaxation, the role of thermal vs. nonthermal electron and phonon scattering on overall electron energy transfer to the phonons remains unclear. In this work, we derive an analytical expression for the electron-phonon coupling factor in a metal that includes contributions from equilibrium and nonequilibrium distributions of electrons. While the contribution from the nonthermal electrons to electron-phonon coupling is non-negligible, the increase in the electron relaxation rates with increasing laser fluence measured by thermoreflectance techniques cannot be accounted for by only considering electron-phonon relaxations. We conclude that electron-electron scattering along with electron-phonon scattering have to be considered simultaneously to correctly predict the transient nature of electron relaxation during and after short-pulsed heating of metals at elevated electron temperatures. Furthermore, for high electron temperature perturbations achieved at high absorbed laser fluences, we show good agreement between our model, which accounts for d-band excitations, and previous experimental data. Our model can be extended to other free electron metals with the knowledge of the density of states of electrons in the metals and considering electronic excitations from non-Fermi surface states.
Effect of electron heating on femtosecond laser-induced coherent acoustic phonons in noble metals
Wang, Jincheng; Guo, Chunlei
2007-05-01
We employ a surface plasmon technique to resolve the dynamics of femtosecond-laser-induced coherent acoustic phonons in noble metals. Clear acoustic oscillations are observed in our experiments. We further study the dependence of the initial phase of the oscillations on pump fluence, and we find that the initial phase decreases linearly with pump fluence. Our model calculations show that hot electrons instantaneously excited by femtosecond pulses contribute to the generation of coherent acoustic phonons in metals.
Confinement of phonon propagation in laser deposited tungsten/polycarbonate multilayers
Döring, Florian; Ulrichs, Henning; Pagel, Sinja; Müller, Markus; Mansurova, Maria; Müller, Matthias; Eberl, Christian; Erichsen, Torben; Huebner, Dennis; Vana, Philipp; Mann, Klaus; Münzenberg, Markus; Krebs, Hans-Ulrich
2016-09-01
Nanoscale multilayer thin films of W and PC (Polycarbonate) show, due to the great difference of the components’ characteristics, fascinating properties for a variety of possible applications and provide an interesting research field, but are hard to fabricate with low layer thicknesses. Because of the great acoustic mismatch between the two materials, such nanoscale structures are promising candidates for new phononic materials, where phonon propagation is strongly reduced. In this article we show for the first time that W/PC-multilayers can indeed be grown with high quality by pulsed laser deposition. We analyzed the polymer properties depending on the laser fluence used for deposition, which enabled us to find best experimental conditions for the fabrication of high-acoustic-mismatch W/PC multilayers. The multilayers were analyzed by fs pump-probe spectroscopy showing that phonon dynamics on the ps time-scale can strongly be tailored by structural design. While already periodic multilayers exhibit strong phonon localization, especially aperiodic structures present outstandingly low phonon propagation properties making such 1D-layered W/PC nano-structures interesting for new phononic applications.
Ultrafast electron diffraction from non-equilibrium phonons in femtosecond laser heated Au films
Energy Technology Data Exchange (ETDEWEB)
Chase, T. [Stanford Institute for Materials and Energy Sciences, SLAC National Accelerator Laboratory, 2575 Sand Hill Road, Menlo Park, California 94025 (United States); Department of Applied Physics, Stanford University, Stanford, California 94305 (United States); Trigo, M.; Reid, A. H.; Dürr, H. A. [Stanford Institute for Materials and Energy Sciences, SLAC National Accelerator Laboratory, 2575 Sand Hill Road, Menlo Park, California 94025 (United States); Li, R.; Vecchione, T.; Shen, X.; Weathersby, S.; Coffee, R.; Hartmann, N.; Wang, X. J. [SLAC National Accelerator Laboratory, 2575 Sand Hill Road, Menlo Park, California 94025 (United States); Reis, D. A. [Stanford Institute for Materials and Energy Sciences, SLAC National Accelerator Laboratory, 2575 Sand Hill Road, Menlo Park, California 94025 (United States); Department of Applied Physics, Stanford University, Stanford, California 94305 (United States); PULSE Institute, SLAC National Accelerator Laboratory, 2575 Sand Hill Road, Menlo Park, California 94025 (United States)
2016-01-25
We use ultrafast electron diffraction to detect the temporal evolution of non-equilibrium phonons in femtosecond laser-excited ultrathin single-crystalline gold films. From the time-dependence of the Debye-Waller factor, we extract a 4.7 ps time-constant for the increase in mean-square atomic displacements. The observed increase in the diffuse scattering intensity demonstrates that the energy transfer from laser-heated electrons to phonon modes near the X and K points in the Au fcc Brillouin zone proceeds with timescales of 2.3 and 2.9 ps, respectively, faster than the Debye-Waller average mean-square displacement.
Mode-selective phonon excitation in gallium nitride using mid-infrared free-electron laser
Kagaya, Muneyuki; Yoshida, Kyohei; Zen, Heishun; Hachiya, Kan; Sagawa, Takashi; Ohgaki, Hideaki
2017-02-01
The single-phonon mode was selectively excited in a solid-state sample. A mid-infrared free-electron laser, which was tuned to the target phonon mode, was irradiated onto a crystal cooled to a cryogenic temperature, where modes other than the intended excitation were suppressed. An A 1(LO) vibrational mode excitation on GaN(0001) face was demonstrated. Anti-Stokes Raman scattering was used to observe the excited vibrational mode, and the appearance and disappearance of the scattering band at the target wavenumber were confirmed to correspond to on and off switching of the pump free-electron laser and were fixed to the sample vibrational mode. The sum-frequency generation signals of the pump and probe lasers overlapped the Raman signals and followed the wavenumber shift of the pump laser.
Iotti, Rita C.; Rossi, Fausto
2013-07-01
The operation of state-of-the-art optoelectronic quantum devices may be significantly affected by the presence of a nonequilibrium quasiparticle population to which the carrier subsystem is unavoidably coupled. This situation is particularly evident in new-generation semiconductor-heterostructure-based quantum emitters, operating both in the mid-infrared as well as in the terahertz (THz) region of the electromagnetic spectrum. In this paper, we present a Monte Carlo-based global kinetic approach, suitable for the investigation of a combined carrier-phonon nonequilibrium dynamics in realistic devices, and discuss its application with a prototypical resonant-phonon THz emitting quantum cascade laser design.
Manipulation of Squeezed Two-Phonon Bound States using Femtosecond Laser Pulses
Directory of Open Access Journals (Sweden)
Nakamura Kazutaka G.
2013-03-01
Full Text Available Two-phonon bound states have been excited exclusively in ZnTe(110 via impulsive stimulated second-order Raman scattering, essentially being squeezed states due to phase coherent excitation of two identical components anticorrelated in the wave vector. By using coherent control technique with a pair of femtosecond laser pulses, the manipulation of squeezed states has been demonstrated in which both the amplitude and lifetime of coherent oscillations of squeezed states are modulated, indicating the feasibility to control the quantum noise and the quantum nature of phonon squeezed states, respectively.
Rapid phase change induced by double picosecond laser pulses and the dynamics of acoustic phonons
Energy Technology Data Exchange (ETDEWEB)
Li, Simian, E-mail: lism1972@qq.com [Hebei Key Laboratory of Optoelectronic Information and Geo-detection Technology, Shijiazhuang University of Economics, Shijiazhuang 050031 (China); State Key Laboratory of Optoelectronic Materials and Technology, School of Physics and Engineering, Sun Yat-Sen University, Guangzhou 510275 (China); Liang, Guangfei [Key Laboratory of High Power Laser Materials, Shanghai Institute of Optics and Fine Mechanics, Chinese Academy of Sciences, Shanghai 201800 (China)
2013-12-02
For a given phase change material and composition, the double laser pulses better than a single pulse for the crystallization process. We investigated the crystallization process in Si{sub 15}Sb{sub 85} thin films induced by double picosecond pulses with constant fluence and variable intervals. The crystallization degree is a function of the intervals of double pump laser pulses. The crystallization time decreased with the increasing of the intervals of the pump pulses. We believe that acoustic phonons play a key role in the crystallization process. - Highlights: • The double pulse crystallization is easier than the single pulse crystallization. • The crystallization is a function of the intervals of double pump laser pulses. • The crystallization time decreases with the increase of the pump pulse intervals. • Acoustic phonons play a key role in the crystallization process.
Far-infrared quantum cascade lasers operating in AlAs phonon Reststrahlen band
Ohtani, K; Süess, M J; Faist, J; Andrews, A M; Zederbauer, T; Detz, H; Schrenk, W; Strasser, G
2016-01-01
We report on the operation of a double metal waveguide far-infrared quantum cascade laser emitting at 28 $\\mu$m, corresponding to the AlAs-like phonon Reststrahlen band. To avoid absorption by AlAs-like optical phonons, the Al-free group-V alloy GaAs$_{0.51}$Sb$_{0.49}$ is used as a barrier layer in the bound-to-continuum based active region. Lasing occurs at a wavelength of 28.3 $\\mu$m, which is the longest wavelength among the quantum cascade lasers operating from mid-infrared to far-infrared. The threshold current density at 50 K is 5.5 kA/cm$^{2}$ and maximum operation temperature is 175 K. We also discuss the feasibility that operation wavelength cover the whole spectral range bridging between mid-infrared and terahertz by choosing suited group III-V materials.
Thermal conductivity and electron-phonon relaxation in a metal heated by a subpicosecond laser pulse
Petrov, Yu. V.; Anisimov, S. I.
2006-06-01
This paper discusses the initial stages of the interaction of subpicosecond laser pulses with metallic targets: the absorption of light, energy transport by electronic thermal conductivity, and electron-phonon relaxation. It is shown that, with moderate surface energy density, hydrodynamic motion begins after the electronic and lattice temperatures equalize. A connection is established between the energy exchange rate between the electrons and the lattice and the electronic thermal conductivity (an analog of the Wiedemann-Franz law).
Electron-phonon nonequilibrium during ultrashort pulsed laser heating of metals
Smith, Andrew Neil
2001-10-01
Ultrashort pulsed lasers have repeatedly been demonstrated as an effective tool for the observation of transport properties on atomistic time and length scales. Accordingly, the number of applications of these types of lasers as diagnostic tools is rapidly increasing. To effectively use these tools, precise knowledge of the energy deposition mechanism is absolutely necessary. The accepted model for ultrashort pulsed laser heating is the ``Two Temperature Model'' which assumes equilibrium electron and phonon distributions that are not in equilibrium with each other. Recently the applicability of the ``Two Temperature Model'' has received some scrutiny for very low and very high intensity application. This model gave rise to the electron-phonon coupling factor, which, when combined with the temperature difference between the two systems, represents the rate of energy transfer for small perturbations in temperature. However, numerous applications use moderate to high intensity ultrashort pulses, which create far more than small perturbations in temperature. In this investigation the temperature dependence of the electron-phonon coupling factor, electron heat capacity, and thermal conductivity are examined for significant changes in the electron temperature. Experimental results are presented for transient thermoreflectance data taken at moderate fluences. A significant discrepancy is apparent between the two temperature model and the experimental data taken on Au. This problem was originally thought to arise from increased electron- phonon coupling for moderate changes in the electron temperature. Investigation into the temperature dependence of the electron-phonon coupling factor did not support this hypothesis. It was discovered that the discrepancy was due to a nonlinear relationship between changes in the electron temperature and changes in reflectance. The incident probe energy used when taking the experimental data was 1.5 eV, which is significantly less than
A phonon scattering assisted injection and extraction based terahertz quantum cascade laser
Dupont, E.; Fathololoumi, S.; Wasilewski, Z. R.; Aers, G.; Laframboise, S. R.; Lindskog, M.; Razavipour, S. G.; Wacker, A.; Ban, D.; Liu, H. C.
2012-04-01
A lasing scheme for terahertz quantum cascade lasers, based on consecutive phonon-photon-phonon emissions per module, is proposed and experimentally demonstrated. The charge transport of the proposed structure is modeled using a rate equation formalism. An optimization code based on a genetic algorithm was developed to find a four-well design in the GaAs/Al0.25Ga0.75As material system that maximizes the product of population inversion and oscillator strength at 150 K. The fabricated devices using Au double-metal waveguides show lasing at 3.2 THz up to 138 K. The electrical characteristics display no sign of differential resistance drop at lasing threshold, which, in conjunction with the low optical power of the device, suggest—thanks to the rate equation model—a slow depopulation rate of the lower lasing state, a hypothesis confirmed by non-equilibrium Green's function calculations.
Breaking the low phonon energy barrier for laser cooling in rare-earth doped hosts
Nemova, Galina; Kashyap, Raman
2011-03-01
A new approach to cool rare earth doped solids with optical super-radiance (SR) is presented. SR is the coherent, sharply directed spontaneous emission of photons by a system excited with a pulsed laser. We consider an Yb3+ doped ZBLAN sample pumped at the wavelength 1015nm with a rectangular pulsed source with a power of ~700W and duration of 20ns. The intensity of the SR is proportional to the square of the number of excited ions. This unique feature of SR permits an increase in the rate of the cooling process in comparison with the traditional laser cooling of the rare earth doped solids with anti-Stokes spontaneous incoherent radiation (fluorescence). This scheme overcomes the limitation of using only low phonon energy glasses for laser cooling.
Enhanced performance of thin-disk lasers by pumping into the zero-phonon line.
Weichelt, Birgit; Voss, Andreas; Abdou Ahmed, Marwan; Graf, Thomas
2012-08-01
Pumping Yb:YAG or Yb:LuAG into the zero-phonon line at 969 nm instead of using the common pump wavelength of 940 nm reduces the heat generation by 32%. In addition to the 3% increase of the Stokes efficiency, this significantly reduces the diffraction losses caused by the thermally induced phase distortions leading to a remarkable increase of the overall efficiency especially of fundamental-mode thin-disk lasers. Using this pumping scheme in an Yb:LuAG thin-disk laser, we achieved 742 W of nearly diffraction limited (M2≈1.5) output power at an unprecedented high optical efficiency of 58.5%. For multimode operation (M2≈15) the maximum optical efficiency of an Yb:YAG thin-disk laser was increased to 72%.
1991-01-01
The concepts of source and quantum action principle are used to produce the phonon Green's function appropriate for an initial phonon vacuum state. An application to the Mossbauer effect is presented.
Energy Technology Data Exchange (ETDEWEB)
Yoshida, Kyohei; Hachiya, Kan; Okumura, Kensuke; Mishima, Kenta; Inukai, Motoharu; Torgasin, Konstantin; Omer, Mohamed [Graduate School of Energy Science, Kyoto University, Yoshida-honmachi, Sakyo-ku, Kyoto 606-8501 (Japan); Sonobe, Taro [Kyoto University Research Administration Office, Kyoto University, Yoshida-honmachi, Sakyo-ku, Kyoto 606-8501 (Japan); Zen, Heishun; Negm, Hani; Kii, Toshiteru; Masuda, Kai; Ohgaki, Hideaki [Institute of Advanced Energy, Kyoto University, Gokasyo, Uji, Kyoto 611-0011 (Japan)
2013-10-28
Mode-selective phonon excitation by a mid-infrared laser (MIR-FEL) is demonstrated via anti-Stokes Raman scattering measurements of 6H-silicon carbide (SiC). Irradiation of SiC with MIR-FEL and a Nd-YAG laser at 14 K produced a peak where the Raman shift corresponds to a photon energy of 119 meV (10.4 μm). This phenomenon is induced by mode-selective phonon excitation through the irradiation of MIR-FEL, whose photon energy corresponds to the photon-absorption of a particular phonon mode.
Energy Technology Data Exchange (ETDEWEB)
Yilbas, B.S., E-mail: bsyilbas@kfupm.edu.sa; Ali, H.
2016-08-15
Short-pulse laser heating of aluminum and silicon thin films pair with presence of a minute vacuum gap in between them is considered and energy transfer across the thin films pair is predicted. The frequency dependent Boltzmann equation is used to predict the phonon intensity distribution along the films pair for three cycles of the repetitive short-pulse laser irradiation on the aluminum film surface. Since the gap size considered is within the Casimir limit, thermal radiation and ballistic phonon contributions to energy transfer across the vacuum gap is incorporated. The laser irradiated field is formulated in line with the Lambert's Beer law and it is considered as the volumetric source in the governing equations of energy transport. In order to assess the phonon intensity distribution in the films pair, equivalent equilibrium temperature is introduced. It is demonstrated that thermal separation of electron and lattice sub-systems in the aluminum film, due to the short-pulse laser irradiation, takes place and electron temperature remains high in the aluminum film while equivalent equilibrium temperature for phonons decays sharply in the close region of the aluminum film interface. This behavior is attributed to the phonon boundary scattering at the interface and the ballistic phonon transfer to the silicon film across the vacuum gap. Energy transfer due to the ballistic phonon contribution is significantly higher than that of the thermal radiation across the vacuum gap.
Makovetskii, D N
2011-01-01
This is a part of an overview of my early studies on nonlinear spin-phonon dynamics in solid state optical-wavelength phonon lasers (phasers) started in 1984. The main goal of this work is a short description and a qualitative analysis of experimental data on low-frequency nonlinear resonances revealed in a nonautonomous ruby phaser. Under phaser pumping modulation near these resonances, an unusual kind of self-organized motions in the ruby spin-phonon system was observed by me in 1984 for the first time. The original technique of optical-wavelength microwave-frequency acoustic stimulated emission (SE) detection and microwave-frequency power spectra (MFPS) analysis was used in these experiments (description of the technique see: D.N.Makovetskii, Cand. Sci. Diss., Kharkov, 1983). The real time evolution of MFPS was studied using this technique at scales up to several hours. The phenomenon of the self-organized periodic alternation of SE phonon modes was experimentally revealed at hyperlow frequencies from abou...
Zhou, Jun; Li, Nianbei; Yang, Ronggui
2015-06-01
The electrons and phonons in metal films after ultra-short pulse laser heating are in highly non-equilibrium states not only between the electrons and the phonons but also within the electrons. An electrohydrodynamics model consisting of the balance equations of electron density, energy density of electrons, and energy density of phonons is derived from the coupled non-equilibrium electron and phonon Boltzmann transport equations to study the nonlinear thermal transport by considering the electron density fluctuation and the transient electric current in metal films, after ultra-short pulse laser heating. The temperature evolution is calculated by the coupled electron and phonon Boltzmann transport equations, the electrohydrodynamics model derived in this work, and the two-temperature model. Different laser pulse durations, film thicknesses, and laser fluences are considered. We find that the two-temperature model overestimates the electron temperature at the front surface of the film and underestimates the damage threshold when the nonlinear thermal transport of electrons is important. The electrohydrodynamics model proposed in this work could be a more accurate prediction tool to study the non-equilibrium electron and phonon transport process than the two-temperature model and it is much easier to be solved than the Boltzmann transport equations.
Tang, Jau
2008-04-01
In this study, we examine the ultrafast structural dynamics of metals induced by a femtosecond laser-heating pulse as probed by time-resolved electron diffraction. Using the two-temperature model and the Grüneisen relationship we calculate the electron temperature, phonon temperature, and impulsive force at each atomic site in the slab. Together with the Fermi-Pasta-Ulam anharmonic chain model we calculate changes of bond distance and the peak shift of Bragg spots or Laue rings. A laser-heated thin slab is shown to exhibit "breathing" standing-wave behavior, with a period equal to the round-trip time for sound wave and a wavelength twice the slab thickness. The peak delay time first increases linearly with the thickness (<70nm for aluminum and <200nm for gold), but becomes less dependent if further thickness increases. Coherent phonon excitation and propagation from the stressed bulk atoms due to impulsive forces as well as the linear thermal expansion due to lattice temperature jump are shown to contribute to the overall structural changes. Differences between these two mechanisms and their dependence on film thickness and other factors are discussed.
Phonon engineering for nanostructures.
Energy Technology Data Exchange (ETDEWEB)
Aubry, Sylvie (Stanford University); Friedmann, Thomas Aquinas; Sullivan, John Patrick; Peebles, Diane Elaine; Hurley, David H. (Idaho National Laboratory); Shinde, Subhash L.; Piekos, Edward Stanley; Emerson, John Allen
2010-01-01
Understanding the physics of phonon transport at small length scales is increasingly important for basic research in nanoelectronics, optoelectronics, nanomechanics, and thermoelectrics. We conducted several studies to develop an understanding of phonon behavior in very small structures. This report describes the modeling, experimental, and fabrication activities used to explore phonon transport across and along material interfaces and through nanopatterned structures. Toward the understanding of phonon transport across interfaces, we computed the Kapitza conductance for {Sigma}29(001) and {Sigma}3(111) interfaces in silicon, fabricated the interfaces in single-crystal silicon substrates, and used picosecond laser pulses to image the thermal waves crossing the interfaces. Toward the understanding of phonon transport along interfaces, we designed and fabricated a unique differential test structure that can measure the proportion of specular to diffuse thermal phonon scattering from silicon surfaces. Phonon-scale simulation of the test ligaments, as well as continuum scale modeling of the complete experiment, confirmed its sensitivity to surface scattering. To further our understanding of phonon transport through nanostructures, we fabricated microscale-patterned structures in diamond thin films.
Energy Technology Data Exchange (ETDEWEB)
Krupke, William F. (Pleasanton, CA); Payne, Stephen A. (Castro Valley, CA); Marshall, Christopher D. (Livermore, CA)
2001-01-01
The invention provides an efficient, compact means of generating blue laser light at a wavelength near .about.493+/-3 nm, based on the use of a laser diode-pumped Yb-doped laser crystal emitting on its zero phonon line (ZPL) resonance transition at a wavelength near .about.986+/-6 nm, whose fundamental infrared output radiation is harmonically doubled into the blue spectral region. The invention is applied to the excitation of biofluorescent dyes (in the .about.490-496 nm spectral region) utilized in flow cytometry, immunoassay, DNA sequencing, and other biofluorescence instruments. The preferred host crystals have strong ZPL fluorecence (laser) transitions lying in the spectral range from .about.980 to .about.992 nm (so that when frequency-doubled, they produce output radiation in the spectral range from 490 to 496 nm). Alternate preferred Yb doped tungstate crystals, such as Yb:KY(WO.sub.4).sub.2, may be configured to lase on the resonant ZPL transition near 981 nm (in lieu of the normal 1025 nm transition). The laser light is then doubled in the blue at 490.5 nm.
1990-01-01
The gap between the nonlocalized lattice-phonon description and the localized Einstein oscillator treatment is filled by transforming the phonon Hamiltonian back to the particle variables. The particle-coordinate, normalized, wave function for the phonon vacuum state is exhibited.
Laser Incident Lessons Learned and Action List
Energy Technology Data Exchange (ETDEWEB)
Yarotski, Dmitry Anatolievitch [Los Alamos National Lab. (LANL), Los Alamos, NM (United States)
2016-02-29
On Thursday November 19, 2015, LANL postdoc received an eye injury from a reflected, nonvisible laser beam (Class 4, pulsed, wavelength 800 nanometer). The setup is configured to split the laser output into two work areas in which qualified operators conduct research experiments. During this incident, the laser output beam was being projected to both experimental work areas, although only one experimental area was actively being used. The second laser beam directed to the second work area was blocked by an inappropriate device (Plexiglas, reflective, non-normal incidence) that reflected substantial portion of the beam toward the first setup. In preparation for the measurements, worker stepped on the stepstool and decided to remove the laser goggles to better see the micrometer readings which were difficult to see due to insufficient lighting. Immediately, he noticed a flash of light in his eye. The operator quickly replaced the laser eye-wear and then, using an infrared viewer, located a stray laser beam being reflected from the plexiglas beam block. The operator did not think he had sustained any injury and continued working. Later that day, however, he noticed a blurry spot in the vision of his left eye. He notified his supervisor on Friday morning, November 20, 2015, and was taken by CINT management to Sandia National Laboratories (SNL) medical facility for evaluation. SNL Medical did not find any abnormalities, but referred the operator to a local ophthalmologist for further evaluation. Further evaluations by the ophthalmologist on November 21 and November 23 identified a small spot of inflammation near the fovea on the retina in his left eye. The ophthalmologist stated that this spot would most likely heal on its own and that the blurry spot on the operator's vision would go away. A follow-up visit was scheduled. The employee was released back to work without restrictions.
Phoenix's Laser Beam in Action on Mars
2008-01-01
[figure removed for brevity, see original site] Click on image to view the animation The Surface Stereo Imager camera aboard NASA's Phoenix Mars Lander acquired a series of images of the laser beam in the Martian night sky. Bright spots in the beam are reflections from ice crystals in the low level ice-fog. The brighter area at the top of the beam is due to enhanced scattering of the laser light in a cloud. The Canadian-built lidar instrument emits pulses of laser light and records what is scattered back. The Phoenix Mission is led by the University of Arizona, Tucson, on behalf of NASA. Project management of the mission is by NASA's Jet Propulsion Laboratory, Pasadena, Calif. Spacecraft development is by Lockheed Martin Space Systems, Denver.
Ultrafast dynamics and laser action of organic semiconductors
Vardeny, Zeev Valy
2009-01-01
Spurred on by extensive research in recent years, organic semiconductors are now used in an array of areas, such as organic light emitting diodes (OLEDs), photovoltaics, and other optoelectronics. In all of these novel applications, the photoexcitations in organic semiconductors play a vital role. Exploring the early stages of photoexcitations that follow photon absorption, Ultrafast Dynamics and Laser Action of Organic Semiconductors presents the latest research investigations on photoexcitation ultrafast dynamics and laser action in pi-conjugated polymer films, solutions, and microcavities.In the first few chapters, the book examines the interplay of charge (polarons) and neutral (excitons) photoexcitations in pi-conjugated polymers, oligomers, and molecular crystals in the time domain of 100 fs-2 ns. Summarizing the state of the art in lasing, the final chapters introduce the phenomenon of laser action in organics and cover the latest optoelectronic applications that use lasing based on a variety of caviti...
Wette, Frederik
1991-01-01
In recent years substantial progress has been made in the detection of surface phonons owing to considerable improvements in inelastic rare gas scattering tech niques and electron energy loss spectroscopy. With these methods it has become possible to measure surface vibrations in a wide energy range for all wave vectors in the two-dimensional Brillouin zone and thus to deduce the complete surface phonon dispersion curves. Inelastic atomic beam scattering and electron energy loss spectroscopy have started to play a role in the study of surface phonons similar to the one played by inelastic neutron scattering in the investigation of bulk phonons in the last thirty years. Detailed comparison between experimen tal results and theoretical studies of inelastic surface scattering and of surface phonons has now become feasible. It is therefore possible to test and to improve the details of interaction models which have been worked out theoretically in the last few decades. At this point we felt that a concise, co...
1990-01-01
An atomic lattice in its ground state is excited by the rapid displacement and release of an atomic constituent. The time dependence of the energy transfer to other constituents is studied by using a phonon dispersion relation that is linear in frequency and propagation vector components.
Phonons with orbital angular momentum
Energy Technology Data Exchange (ETDEWEB)
Ayub, M. K. [Theoretical Plasma Physics Division, PINSTECH, P. O. Nilore, Islamabad (Pakistan); National Centre for Physics, Shahdra Valley Road, Quaid-i-Azam University Campus, Islamabad 44000 (Pakistan); Ali, S. [National Centre for Physics, Shahdra Valley Road, Quaid-i-Azam University Campus, Islamabad 44000 (Pakistan); Mendonca, J. T. [IPFN, Instituto Superior Tecnico, Av. Rovisco Pais 1, 1049-001 Lisboa (Portugal)
2011-10-15
Ion accoustic waves or phonon modes are studied with orbital angular momentum (OAM) in an unmagnetized collissionless uniform plasma, whose constituents are the Boltzmann electrons and inertial ions. For this purpose, we have employed the fluid equations to obtain a paraxial equation in terms of ion density perturbations and discussed its Gaussian beam and Laguerre-Gauss (LG) beam solutions. Furthermore, an approximate solution for the electrostatic potential problem is presented, allowing to express the components of the electric field in terms of LG potential perturbations. The energy flux due to phonons is also calculated and the corresponding OAM is derived. Numerically, it is shown that the parameters such as azimuthal angle, radial and angular mode numbers, and beam waist, strongly modify the profiles of the phonon LG potential. The present results should be helpful in understanding the phonon mode excitations produced by Brillouin backscattering of laser beams in a uniform plasma.
Phonon manipulation with phononic crystals.
Energy Technology Data Exchange (ETDEWEB)
Kim Bongsang; Hopkins, Patrick Edward; Leseman, Zayd C.; Goettler, Drew F.; Su, Mehmet F. (University of New Mexico, Albuquerque, NM); El-Kady, Ihab Fathy; Reinke, Charles M.; Olsson, Roy H., III
2012-01-01
In this work, we demonstrated engineered modification of propagation of thermal phonons, i.e. at THz frequencies, using phononic crystals. This work combined theoretical work at Sandia National Laboratories, the University of New Mexico, the University of Colorado Boulder, and Carnegie Mellon University; the MESA fabrication facilities at Sandia; and the microfabrication facilities at UNM to produce world-leading control of phonon propagation in silicon at frequencies up to 3 THz. These efforts culminated in a dramatic reduction in the thermal conductivity of silicon using phononic crystals by a factor of almost 30 as compared with the bulk value, and about 6 as compared with an unpatterned slab of the same thickness. This work represents a revolutionary advance in the engineering of thermoelectric materials for optimal, high-ZT performance. We have demonstrated the significant reduction of the thermal conductivity of silicon using phononic crystal structuring using MEMS-compatible fabrication techniques and in a planar platform that is amenable to integration with typical microelectronic systems. The measured reduction in thermal conductivity as compared to bulk silicon was about a factor of 20 in the cross-plane direction [26], and a factor of 6 in the in-plane direction. Since the electrical conductivity was only reduced by a corresponding factor of about 3 due to the removal of conductive material (i.e., porosity), and the Seebeck coefficient should remain constant as an intrinsic material property, this corresponds to an effective enhancement in ZT by a factor of 2. Given the number of papers in literature devoted to only a small, incremental change in ZT, the ability to boost the ZT of a material by a factor of 2 simply by reducing thermal conductivity is groundbreaking. The results in this work were obtained using silicon, a material that has benefitted from enormous interest in the microelectronics industry and that has a fairly large thermoelectric power
"Social Laser": Action Amplification by Stimulated Emission of Social Energy
Khrennikov, Andrei
2015-01-01
The problem of the "explanation" of recent social explosions, especially in the Middle East, but also in Southern Europe and the USA, have been debated actively in the social and political literature. We can mention the contributions of P. Mason, F. Fukuyama, E. Schmidt and J. Cohen, I. Krastev to this debate. We point out that the diversity of opinions and conclusions is really amazing. At the moment, there is no consistent and commonly acceptable theory of these phenomena. We present a model of social explosions based on a novel approach for the description of social processes, namely, the quantum-like approach. Here quantum theory is treated simply as an operational formalism - without any direct relation to physics. We explore the quantum-like laser model to describe the possibility of Action Amplification by Stimulated Emission of Social Energy (ASE).
Excitons, polarons, and laser action in poly(p-phenylene vinylene) films
Österbacka, R.; Wohlgenannt, M.; Shkunov, M.; Chinn, D.; Vardeny, Z. V.
2003-05-01
onset at 2.4 eV. The photoluminescence spectrum is well structured, showing five phonon side bands with 190 meV separation. We have also studied laser action in PPV thin films and microcavities such as microrings and microdisks. The effective gain spectrum is calculated and the estimated threshold excitation intensity for laser action for the 0-1 transition is found to be in good agreement with the data, with an estimated exciton density of 2×1018 cm-3. Lasing from microring devices shows several narrow waveguide modes, with intermode spacing of 0.45 nm that corresponds to an effective mode refractive index, neff=1.45. The spectral width of the laser modes is resolution limited and gives a lower estimate of the cavity quality factor, Q. For microrings we found Q>5000, which is limited by self-absorption in the polymer film.
El-Kady, Ihab F.; Olsson, Roy H.
2012-01-10
Phononic crystals that have the ability to modify and control the thermal black body phonon distribution and the phonon component of heat transport in a solid. In particular, the thermal conductivity and heat capacity can be modified by altering the phonon density of states in a phononic crystal. The present invention is directed to phononic crystal devices and materials such as radio frequency (RF) tags powered from ambient heat, dielectrics with extremely low thermal conductivity, thermoelectric materials with a higher ratio of electrical-to-thermal conductivity, materials with phononically engineered heat capacity, phononic crystal waveguides that enable accelerated cooling, and a variety of low temperature application devices.
Phononic High Harmonic Generation
Ganesan, Adarsh; Seshia, Ashwin A
2016-01-01
This paper reports the first experimental evidence for phononic low-order to high-order harmonic conversion leading to high harmonic generation. Similar to parametric resonance, phononic high harmonic generation is also mediated by a threshold dependent instability of a driven phonon mode. Once the threshold for instability is met, a cascade of harmonic generation processes is triggered. Firstly, the up-conversion of first harmonic phonons into second harmonic phonons is established. Subsequently, the down-conversion of second harmonic phonons into first harmonic phonons and conversion of first and second harmonic phonons into third harmonic phonons occur. On the similar lines, an eventual conversion of third harmonic phonons to high orders is also observed to commence. This surprising physical pathway for phononic low-order to high-order harmonic conversion may find general relevance to other physical systems.
Random laser action with coherent feedback via second-harmonic generation
Qiao, Yanqi; Cai, Zengyan; Chen, Xianfeng
2016-01-01
The random laser action with coherent feedback by second-harmonic generation (SHG) was experimentally demonstrated in this paper. Compared with the conventional random laser action based on photoluminescence effect, which needs strong photoresponse in the active medium and has a fixed response waveband due to the inherent energy level structure of the material, this random SHG laser action indicates a possible confinement of the nonlinear signal with ring cavities and widens the response waveband due to the flexible frequency conversion in nonlinear process. The combination of coherent random laser and nonlinear optics will provide us another possible way to break phase-matching limitations, with fiber or feedback-based wavefront shaping method to transmit the emission signal directionally. This work suggests potential applications in band-tunable random laser, phase-matching-free nonlinear optics and even brings in new consideration about random nonlinear optics (RNO).
Epidermal Laser Stimulation of Action Potentials in the Frog Sciatic Nerve
2008-10-01
Laser Stimulation of Action Potentials in the Frog Sciatic Nerve Nichole M. Jindra Robert J. Thomas Human Effectiveness Directorate Directed...in the Frog Sciatic Nerve 5b. GRANT NUMBER 5c. PROGRAM ELEMENT NUMBER 62202F 6. AUTHOR(S) .Nichole M. Jindra, Robert J. Thomas, Douglas N...Alan Rice 14. ABSTRACT Measurements of laser stimulated action potentials in the sciatic nerve of leopard frogs (Rana pipiens) were made using
Nonequilibrium heating and cooling of metals under action of supershort laser pulse
Libenson, Mikhail N.
2001-06-01
It is considered photo-excitation, non-equilibrium heating and thermal after-action induced by super-short laser pluses interacting with metals. It is shown that classical model of thermal laser-induced destruction of metals should be corrected in the case when pulse duration is much less than characteristic time of energy transfer from electrons to the lattice. In particular, possible important role of laser- induced electric-physical processes should be taken into account.
Manipulation of Phonons with Phononic Crystals
Energy Technology Data Exchange (ETDEWEB)
Leseman, Zayd Chad [Univ. of New Mexico, Albuquerque, NM (United States)
2015-07-09
There were three research goals associated with this project. First, was to experimentally demonstrate phonon spectrum control at THz frequencies using Phononic Crystals (PnCs), i.e. demonstrate coherent phonon scattering with PnCs. Second, was to experimentally demonstrate analog PnC circuitry components at GHz frequencies. The final research goal was to gain a fundamental understanding of phonon interaction using computational methods. As a result of this work, 7 journal papers have been published, 1 patent awarded, 14 conference presentations given, 4 conference publications, and 2 poster presentations given.
Two-Dimensional Phononic Crystals: Disorder Matters.
Wagner, Markus R; Graczykowski, Bartlomiej; Reparaz, Juan Sebastian; El Sachat, Alexandros; Sledzinska, Marianna; Alzina, Francesc; Sotomayor Torres, Clivia M
2016-09-14
The design and fabrication of phononic crystals (PnCs) hold the key to control the propagation of heat and sound at the nanoscale. However, there is a lack of experimental studies addressing the impact of order/disorder on the phononic properties of PnCs. Here, we present a comparative investigation of the influence of disorder on the hypersonic and thermal properties of two-dimensional PnCs. PnCs of ordered and disordered lattices are fabricated of circular holes with equal filling fractions in free-standing Si membranes. Ultrafast pump and probe spectroscopy (asynchronous optical sampling) and Raman thermometry based on a novel two-laser approach are used to study the phononic properties in the gigahertz (GHz) and terahertz (THz) regime, respectively. Finite element method simulations of the phonon dispersion relation and three-dimensional displacement fields furthermore enable the unique identification of the different hypersonic vibrations. The increase of surface roughness and the introduction of short-range disorder are shown to modify the phonon dispersion and phonon coherence in the hypersonic (GHz) range without affecting the room-temperature thermal conductivity. On the basis of these findings, we suggest a criteria for predicting phonon coherence as a function of roughness and disorder.
Nanoscale pillar hypersonic surface phononic crystals
Yudistira, D.; Boes, A.; Graczykowski, B.; Alzina, F.; Yeo, L. Y.; Sotomayor Torres, C. M.; Mitchell, A.
2016-09-01
We report on nanoscale pillar-based hypersonic phononic crystals in single crystal Z-cut lithium niobate. The phononic crystal is formed by a two-dimensional periodic array of nearly cylindrical nanopillars 240 nm in diameter and 225 nm in height, arranged in a triangular lattice with a 300-nm lattice constant. The nanopillars are fabricated by the recently introduced nanodomain engineering via laser irradiation of patterned chrome followed by wet etching. Numerical simulations and direct measurements using Brillouin light scattering confirm the simultaneous existence of nonradiative complete surface phononic band gaps. The band gaps are found below the sound line at hypersonic frequencies in the range 2-7 GHz, formed from local resonances and Bragg scattering. These hypersonic structures are realized directly in the piezoelectric material lithium niobate enabling phonon manipulation at significantly higher frequencies than previously possible with this platform, opening new opportunities for many applications in plasmonic, optomechanic, microfluidic, and thermal engineering.
Length-scale dependent phonon interactions
Srivastava, Gyaneshwar
2014-01-01
This book presents a comprehensive description of phonons and their interactions in systems with different dimensions and length scales. Internationally-recognized leaders describe theories and measurements of phonon interactions in relation to the design of materials with exotic properties such as metamaterials, nano-mechanical systems, next-generation electronic, photonic, and acoustic devices, energy harvesting, optical information storage, and applications of phonon lasers in a variety of fields. The emergence of techniques for control of semiconductor properties and geometry has enabled engineers to design structures in which functionality is derived from controlling electron behavior. As manufacturing techniques have greatly expanded the list of available materials and the range of attainable length scales, similar opportunities now exist for designing devices whose functionality is derived from controlling phonon behavior. However, progress in this area is hampered by gaps in our knowledge of phono...
Multiple Quantum Wells for P T -Symmetric Phononic Crystals
Poshakinskiy, A. V.; Poddubny, A. N.; Fainstein, A.
2016-11-01
We demonstrate that the parity-time symmetry for sound is realized in laser-pumped multiple-quantum-well structures. Breaking of the parity-time symmetry for the phonons with wave vectors corresponding to the Bragg condition makes the structure a highly selective acoustic wave amplifier. Single-mode distributed feedback phonon lasing is predicted for structures with realistic parameters.
Random Laser Action in Nd:YAG Crystal Powder
Directory of Open Access Journals (Sweden)
Jon Azkargorta
2016-05-01
Full Text Available This work explores the room temperature random stimulated emission at 1.064 μm of a Nd:YAG crystal powder (Neodymium-doped yttrium aluminum garnet in a very simple pump configuration with no assistance from an internal mirror. The laser threshold energy as a function of pump beam area and pump wavelength has been measured, as well as the temporal dynamics of emission pulses. The absolute energy of stimulated emission and the absolute laser slope efficiency have been measured by using a method proposed by the authors. The results show a surprising high efficiency that takes the low Nd3+ ion concentration of the crystal powder into account.
Demonstration of laser action in a pseudo-random medium
Yang, Jin-Kyu; Boriskina, Svetlana V.; Noh, Heeso; Rooks, Michael J.; Solomon, Glenn S.; Dal Negro, Luca; Cao, Hui
2010-08-01
We demonstrated lasing in localized optical resonances of deterministic aperiodic structures with pseudo-random morphologies. The localized lasing modes in the Rudin-Shapiro arrays of air nanoholes in GaAs membranes occur at reproducible spatial locations and their frequencies are only slightly affected by the structural fluctuations in different samples. Numerical study on the resonances of the passive systems and optical imaging of lasing modes enabled us to interpret the observed lasing behavior in terms of distinctive localized resonances in the two-dimensional Rudin- Shapiro structures. The deterministic aperiodic media with controllable structural and optical properties provide a novel platform, alternative to random lasers and different from photonic crystals lasers, for the engineering of multi-frequency coherent light sources suitable for technological integration.
Phonon counting and intensity interferometry of a nanomechanical resonator
Cohen, Justin D; MacCabe, Gregory S; Groblacher, Simon; Safavi-Naeini, Amir H; Marsili, Francesco; Shaw, Matthew D; Painter, Oskar
2014-01-01
Using an optical probe along with single photon detection we have performed effective phonon counting measurements of the acoustic emission and absorption processes in a nanomechanical resonator. Applying these measurements in a Hanbury Brown and Twiss set-up, phonon correlations of the nanomechanical resonator are explored from below to above threshold of a parametric instability leading to self-oscillation of the resonator. Discussion of the results in terms of a "phonon laser", and analysis of the sensitivity of the phonon counting technique are presented.
Coherent radial-breathing-like phonons in graphene nanoribbons
Sanders, G. D.; Nugraha, A. R. T.; Saito, R.; Stanton, C. J.
2012-05-01
We have developed a microscopic theory for the generation and detection of coherent phonons in armchair and zigzag graphene nanoribbons using an extended tight-binding model for the electronic states and a valence force field model for the phonons. The coherent phonon amplitudes satisfy a driven oscillator equation with the driving term depending on photoexcited carrier density. We examine the coherent phonon radial-breathing-like mode amplitudes as a function of excitation energies and nanoribbon types. For photoexcitation near the optical absorption edge the coherent phonon driving term for the radial-breathing-like mode is much larger for zigzag nanoribbons where transitions between localized edge states provide the dominant contribution to the coherent phonon driving term. Using an effective mass theory, we explain how the armchair nanoribbon width changes in response to laser excitation.
Gorishnyy, T; Ullal, C K; Maldovan, M; Fytas, G; Thomas, E L
2005-03-25
In this Letter we propose the use of hypersonic phononic crystals to control the emission and propagation of high frequency phonons. We report the fabrication of high quality, single crystalline hypersonic crystals using interference lithography and show that direct measurement of their phononic band structure is possible with Brillouin light scattering. Numerical calculations are employed to explain the nature of the observed propagation modes. This work lays the foundation for experimental studies of hypersonic crystals and, more generally, phonon-dependent processes in nanostructures.
Long-time correlated quantum dynamics of phonon cooling
Carlig, Sergiu; Macovei, Mihai A.
2014-01-01
We investigate the steady-state cooling dynamics of vibrational degrees of freedom related to a nanomechanical oscillator coupled with a laser-pumped quantum dot in an optical resonator. Correlations between phonon-cooling and quantum-dot photon emission processes occur respectively when a photon laser absorption together with a vibrational phonon absorption is followed by photon emission in the optical resonator. Therefore, the detection of photons generated in the cavity mode concomitantly ...
Hyperfine phononic frequency comb
Ganesan, Adarsh; Seshia, Ashwin A
2016-01-01
Optical frequency combs [1-8] have resulted in significant advances in optical frequency metrology and found wide application to precise physical measurements [1-4, 9] and molecular fingerprinting [8]. A direct analogue of frequency combs in the phononic or acoustic domain has not been reported to date. In this letter, we report the first clear experimental evidence for a phononic frequency comb. In contrast to the Kerr nonlinearity [10] in optical frequency comb formation, the phononic frequency comb is generated through the intrinsic coupling of a driven phonon mode with an auto-parametrically excited sub-harmonic mode [16]. Through systematic experiments at different drive frequencies and amplitudes, we portray the well-connected process of phononic frequency comb formation and define attributes to control the features [17-18] associated with comb formation in such a system. Further, the interplay between these nonlinear resonances and the well-known Duffing phenomenon [12-14] is also observed. The present...
Heat-Pipe Bismuth Laser; Examination of Laser Action at 4722A in Bismuth Vapor
1976-11-01
transitions in other atomic vapors. 13. MODELING OF THE INITIAL BREAKDOWN PROCESS During the initial nanosecond after the fast thyratron switch closes suddenly...lasers computer modeling , laser kin etics bismuth vapor pressure and composition excitation cross sections bismuth dim ers e8ifn.eividienibbek 2Q...P3 / 2 " p $3/4 transi- 3/4 3/2 tion probability is at least a factor of 20 too low. Continuation of the computer modeling begun in this study could
Plasma acceleration and cooling by strong laser field due to the action of radiation reaction force.
Berezhiani, V I; Mahajan, S M; Yoshida, Z
2008-12-01
It is shown that for super intense laser pulses propagating in a hot plasma, the action of the radiation reaction force (appropriately incorporated into the equations of motion) causes strong bulk plasma motion with the kinetic energy raised even to relativistic values; the increase in bulk energy is accompanied by a corresponding cooling (intense cooling) of the plasma. The effects are demonstrated through explicit analytical calculations.
Ivanov, Krill I.; Titorenko, Vladimir A.; Shoub, Gennady M.; Lepilin, Alexander V.; Ovchinnikov, Ilya S.; Mischenko, Oksana S.; Tuchin, Valery V.
2000-03-01
We have studied photodynamic action of He-Ne laser radiation on cultures of Staphylococcus (strain 209 P), Streptococcus anhaemolyticus, and total microflora of dental deposit been sensitized by methylene blue. The concentration of the dye was varied from 0.001% to 0.1%, radiation power density was 100 mW/cm2. Irradiated strain was put into thermostat for 24 hours, then the number of colonies was counted and analyzed.
Origin of coherent G -band phonon spectra in single-wall carbon nanotubes
Nugraha, A. R. T.; Hasdeo, E. H.; Sanders, G. D.; Stanton, C. J.; Saito, R.
2015-01-01
Coherent phonons in single-wall carbon nanotubes (SWNTs) are observed as oscillations of the differential absorption coefficient as a function of time by means of pump-probe spectroscopy. For the radial breathing mode (RBM) of a SWNT, the coherent phonon signal is understood to be a result of the modulated diameter-dependent energy gaps due to the coherent RBM phonon oscillations. However, this mechanism might not be the dominant contribution to other phonon modes in the SWNT. In particular, for the G -band phonons, which correspond to bond-stretching motions, we find that the modulation of the interatomic optical dipole (electron-photon) matrix element gives rise to a strong coherent G -band phonon intensity comparable to the coherent RBM phonon intensity. We also further discuss the dependence of coherent G -band and RBM phonon amplitudes on the laser excitation pulse width.
Phonon-induced polariton superlattices
DEFF Research Database (Denmark)
de Lima, Jr., M. M.; Poel, Mike van der; Santos, P. V.;
2006-01-01
We show that the coherent interaction between microcavity polaritons and externally stimulated acoustic phonons forms a tunable polariton superlattice with a folded energy dispersion determined by the phonon population and wavelength. Under high phonon concentration, the strong confinement of the...... of the optical and excitonic polariton components in the phonon potential creates weakly coupled polariton wires with a virtually flat energy dispersion....
Slow light and slow acoustic phonons in optophononic resonators
Villafañe, V.; Soubelet, P.; Bruchhausen, A. E.; Lanzillotti-Kimura, N. D.; Jusserand, B.; Lemaître, A.; Fainstein, A.
2016-11-01
Slow and confined light have been exploited in optoelectronics to enhance light-matter interactions. Here we describe the GaAs/AlAs semiconductor microcavity as a device that, depending on the excitation conditions, either confines or slows down both light and optically generated acoustic phonons. The localization of photons and phonons in the same place of space amplifies optomechanical processes. Picosecond laser pulses are used to study through time-resolved reflectivity experiments the coupling between photons and both confined and slow acoustic phonons when the laser is tuned either with the cavity (confined) optical mode or with the stop-band edge (slow) optical modes. A model that fully takes into account the modified propagation of the acoustic phonons and light in these resonant structures is used to describe the laser detuning dependence of the coherently generated phonon spectra and amplitude under these different modes of laser excitation. We observe that confined light couples only to confined mechanical vibrations, while slow light can generate both confined and slow coherent vibrations. A strong enhancement of the optomechanical coupling using confined photons and vibrations, and also with properly designed slow photon and phonon modes, is demonstrated. The prospects for the use of these optoelectronic devices in confined and slow optomechanics are addressed.
Institute of Scientific and Technical Information of China (English)
O. Rafil; M. Tamine; B. Bourahla; R. Tigrine; S. Amoudache; A. Khater
2006-01-01
We have theoretically resolved phonon excitations in quasi-two-dimensional organic crystals of polyacenic semiconductor material which may be obtained by the pyrolytic treatment of phenol-formaldehyde resin. A model for studying the dynamical properties using three polyacene chains is proposed with the aim to present the vibrational properties of this structure. It employs the formalism of solid states in two dimensions which admit phonons. A simulation process of the two-dimensional lattice structure shows that elastic waves may explain the existence of vibrational modes in the frequency range 100-400 cm-1. The presence of acoustic and optical like phonons is discussed in terms of the elastic force constants. A hyperfine resonance structure is obtained. It allows the analysis of the dynamical evolution in thin films of polyacene. It is found that the behavior of the phonon density of states exhibits resonance between modes in the structure.
Birefringent phononic structures
Directory of Open Access Journals (Sweden)
I. E. Psarobas
2014-12-01
Full Text Available Within the framework of elastic anisotropy, caused in a phononic crystal due to low crystallographic symmetry, we adopt a model structure, already introduced in the case of photonic metamaterials, and by analogy, we study the effect of birefringence and acoustical activity in a phononic crystal. In particular, we investigate its low-frequency behavior and comment on the factors which determine chirality by reference to this model.
Acceleration of electrons under the action of petawatt-class laser pulses onto foam targets
Pugachev, L. P.; Andreev, N. E.; Levashov, P. R.; Rosmej, O. N.
2016-09-01
Optimization study for future experiments on interaction of petawatt laser pulses with foam targets was done by 3D PIC simulations. Densities in the range 0.5nc-nc and thicknesses in the range 100 - 500 μm of the targets were considered corresponding to those which are currently available. It is shown that heating of electrons mainly occurs under the action of the ponderomotive force of a laser pulse in which amplitude increases up to three times because of self-focusing effect in underdense plasma. Accelerated electrons gain additional energy directly from the high-frequency laser field at the betatron resonance in the emerging plasma density channels. For thicker targets a higher number of electrons with higher energies are obtained. The narrowing of the angular distribution of electrons for thicker targets is explained by acceleration in multiple narrow filaments. Obtained energies of accelerated electrons can be approximated by Maxwell distribution with the temperature 8.5 MeV. The charge carried by electrons with energies higher than 30 MeV is about 30 nC, that is 3-4 order of magnitude higher than the charge predicted by the ponderomotive scaling for the incident laser amplitude.
2005-10-31
Quantum Cascade Laser Fabrication 102 6.3.3.1 Mask Design 102 6.3.3.2 Ohmic Contacts and Device Resistance 102 6.4 Thermo-Wax-Jet Rapid Prototype Photonic...the Photonic Center to those of (A) (G2959) grown at Wright-Pat. 101 6.3.3 Terahertz Quantum Cascade Laser Fabrication 6.3.3.1 Mask design Our laser
Random laser action from a natural flexible biomembrane-based device
Liu, Xiyun; Li, Tingshuai; Yi, Tao; Wang, Chuanke; Li, Jin; Xu, Min; Huang, Dengfeng; Liu, Shenye; Jiang, Shaoen; Ding, Yongkun
2016-07-01
Incoherent random lasing action in flexible eggshell membranes infiltrated with rhodamine 6G laser dyes is demonstrated. Laser radiation is achieved by exciting samples with 1-ns pulses at 526 nm. A threshold of 58 μJ/pulse is measured for the samples. The minimum threshold decreases to 35 μJ/pulse after the sample is coated with gold nanoparticles using a magnetron sputtering technique. The peaks of emission spectra are observed to redshift from 576 to 596 nm as dye concentration rises from 0.03 to 0.6 wt%. A linewidth of approximately 5 nm is obtained for most samples. This study is expected to offer a new way to induce lasing emission using biological microfibrils, and enriches basic knowledge of biophotonics.
Dejneka, S. Y.
1997-12-01
The study of a possible cytotoxic effect of different doses of low-insensitive laser radiation and protective action of low-intensive laser radiation relative to the toxic effect of metals was carried out by means of the alternative method of investigation in vitro on cell cultura Hela. It was established that the investigated doses of low-intensive laser radiation had not produced any toxic effect on cell culture Hela, so the mentioned doses were not cytotoxic. It was revealed that laser radiation reduced the level of the cytotoxic effect of the studied metal salts on the cell culture, and possessed the protective action against the toxic effect of metals. This action has a clear-cut dose- related character.
Phonon waveguides for electromechanical circuits
Hatanaka, D.; Mahboob, I.; Onomitsu, K.; Yamaguchi, H.
2014-07-01
Nanoelectromechanical systems (NEMS), utilizing localized mechanical vibrations, have found application in sensors, signal processors and in the study of macroscopic quantum mechanics. The integration of multiple mechanical elements via electrical or optical means remains a challenge in the realization of NEMS circuits. Here, we develop a phonon waveguide using a one-dimensional array of suspended membranes that offers purely mechanical means to integrate isolated NEMS resonators. We demonstrate that the phonon waveguide can support and guide mechanical vibrations and that the periodic membrane arrangement also creates a phonon bandgap that enables control of the phonon propagation velocity. Furthermore, embedding a phonon cavity into the phonon waveguide allows mobile mechanical vibrations to be dynamically switched or transferred from the waveguide to the cavity, thereby illustrating the viability of waveguide-resonator coupling. These highly functional traits of the phonon waveguide architecture exhibit all the components necessary to permit the realization of all-phononic NEMS circuits.
Perrin, Bernard
2007-06-01
The conference PHONONS 2007 was held 15-20 July 2007 in the Conservatoire National des Arts et Métiers (CNAM) Paris, France. CNAM is a college of higher technology for training students in the application of science to industry, founded by Henri Grégoire in 1794. This was the 12th International Conference on Phonon Scattering in Condensed Matter. This international conference series, held every 3 years, started in France at Sainte-Maxime in 1972. It was then followed by meetings at Nottingham (1975), Providence (1979), Stuttgart (1983), Urbana-Champaign (1986), Heidelberg (1989), Ithaca (1992), Sapporo (1995), Lancaster (1998), Dartmouth (2001) and St Petersburg (2004). PHONONS 2007 was attended by 346 delegates from 37 different countries as follows: France 120, Japan 45, Germany 25, USA 25, Russia 21, Italy 13, Poland 9, UK 9, Canada 7, The Netherlands 7, Finland 6, Spain 6, Taiwan 6, Greece 4, India 4, Israel 4, Ukraine 4, Serbia 3, South Africa 3, Argentina 2, Belgium 2, China 2, Iran 2, Korea 2, Romania 2, Switzerland 2, and one each from Belarus, Bosnia-Herzegovina, Brazil, Bulgaria, Egypt, Estonia, Mexico, Moldova, Morocco, Saudi Arabia, Turkey. There were 5 plenary lectures, 14 invited talks and 84 oral contributions; 225 posters were presented during three poster sessions. The first plenary lecture was given by H J Maris who presented fascinating movies featuring the motion of a single electron in liquid helium. Robert Blick gave us a review on the new possibilities afforded by nanotechnology to design nano-electomechanical systems (NEMS) and the way to use them to study elementary and fundamental processes. The growing interest for phonon transport studies in nanostructured materials was demonstrated by Arun Majumdar. Andrey Akimov described how ultrafast acoustic solitons can monitor the optical properties of quantum wells. Finally, Maurice Chapellier told us how phonons can help tracking dark matter. These 328 presentations gave rise to 185 articles
PHONONS IN INTRINSIC JOSEPHSON SYSTEMS
Energy Technology Data Exchange (ETDEWEB)
C. PREIS; K. SCHMALZL; ET AL
2000-10-01
Subgap structures in the I-V curves of layered superconductors are explained by the excitation of phonons by Josephson oscillations. In the presence of a magnetic field applied parallel to the layers additional structures due to fluxon motion appear. Their coupling with phonons is investigated theoretically and a shift of the phonon resonances in strong magnetic fields is predicted.
Phonons in Ge/Si superlattices with Ge quantum dots
Milekhin, A G; Pchelyakov, O P; Schulze, S; Zahn, D R T
2001-01-01
Ge/Si superlattices with Ge quantum dots obtained by means of molecular-beam epitaxy were investigated by means of light Raman scattering under resonance conditions. These structures are shown to have oscillation properties of both two-dimensional and zero-dimensional objects. Within spectrum low-frequency range one observes twisted acoustic phonons (up to 15 order) typical for planar superlattices. Lines of acoustic phonons are overlapped with a wide band of continuous emission. Analysis of frequencies of Ge and Ge-Si optical phonons shows that Ge quantum dots are pseudoamorphous ones and mixing of Ge and Si atoms is a negligible one. One detected low-frequency shift of longitudinal optical phonons at laser excitation energy increase (2.54-2.71 eV)
Phononic crystals fundamentals and applications
Adibi, Ali
2016-01-01
This book provides an in-depth analysis as well as an overview of phononic crystals. This book discusses numerous techniques for the analysis of phononic crystals and covers, among other material, sonic and ultrasonic structures, hypersonic planar structures and their characterization, and novel applications of phononic crystals. This is an ideal book for those working with micro and nanotechnology, MEMS (microelectromechanical systems), and acoustic devices. This book also: Presents an introduction to the fundamentals and properties of phononic crystals Covers simulation techniques for the analysis of phononic crystals Discusses sonic and ultrasonic, hypersonic and planar, and three-dimensional phononic crystal structures Illustrates how phononic crystal structures are being deployed in communication systems and sensing systems.
Suppression of nonlinear phonon relaxation in Yb:YAG thin disk via zero phonon line pumping.
Smrž, Martin; Miura, Taisuke; Chyla, Michal; Nagisetty, Siva; Novák, Ondřej; Endo, Akira; Mocek, Tomáš
2014-08-15
A quantitative comparison of conventional absorption line (940 nm) pumping and zero phonon line (ZPL) (969 nm) pumping of a Yb:YAG thin disk laser is reported. Characteristics of an output beam profile, surface temperature, and deformation of a thin disk under the different pump wavelengths are evaluated. We found that a nonlinear phonon relaxation (NPR) of the excited state in Yb:YAG, which induces nonlinear temperature rise and large aspheric deformation, did not appear in the case of a ZPL pumped Yb:YAG thin disk. This means that the advantage of ZPL pumping is not only the reduction of quantum defect but also the suppression of NPR. The latter effect is more important for high power lasers.
Laser phase noise effects on the dynamics of optomechanical resonators
Phelps, Gregory A
2010-01-01
We investigate theoretically the influence of laser phase noise on the cooling and heating of a generic cavity optomechanical system. We derive the back-action damping and heating rates and the mechanical frequency shift of the radiation pressure-driven oscillating mirror, and derive the minimum phonon occupation number for small laser linewidths. We find that in practice laser phase noise does not pose serious limitations to ground state cooling. We then consider the effects of laser phase noise in a parametric cavity driving scheme that minimizes the back-action heating of one of the quadratures of the mechanical oscillator motion. Laser linewidths narrow compared to the decay rate of the cavity field will not pose any problems in an experimental setting, but broader linewidths limit the practicality of this back-action evasion method.
The heat-pipe resembling action of boiling bubbles in endovenous laser ablation.
van der Geld, Cees W M; van den Bos, Renate R; van Ruijven, Peter W M; Nijsten, Tamar; Neumann, H A Martino; van Gemert, Martin J C
2010-11-01
Endovenous laser ablation (EVLA) produces boiling bubbles emerging from pores within the hot fiber tip and traveling over a distal length of about 20 mm before condensing. This evaporation-condensation mechanism makes the vein act like a heat pipe, where very efficient heat transport maintains a constant temperature, the saturation temperature of 100 degrees C, over the volume where these non-condensing bubbles exist. During EVLA the above-mentioned observations indicate that a venous cylindrical volume with a length of about 20 mm is kept at 100 degrees C. Pullback velocities of a few mm/s then cause at least the upper part of the treated vein wall to remain close to 100 degrees C for a time sufficient to cause irreversible injury. In conclusion, we propose that the mechanism of action of boiling bubbles during EVLA is an efficient heat-pipe resembling way of heating of the vein wall.
Absence of phase-dependent noise in time-domain reflectivity studies of impulsively excited phonons
Hussain, A.
2010-06-17
There have been several reports of phase-dependent noise in time-domain reflectivity studies of optical phonons excited by femtosecond laser pulses in semiconductors, semimetals, and superconductors. It was suggested that such behavior is associated with the creation of squeezed phonon states although there is no theoretical model that directly supports such a proposal. We have experimentally re-examined the studies of phonons in bismuth and gallium arsenide, and find no evidence of any phase-dependent noise signature associated with the phonons. We place an upper limit on any such noise at least 40–50 dB lower than previously reported.
Yu, Si-Yuan; Sun, Xiao-Chen; Ni, Xu; Wang, Qing; Yan, Xue-Jun; He, Cheng; Liu, Xiao-Ping; Feng, Liang; Lu, Ming-Hui; Chen, Yan-Feng
2016-12-01
Strategic manipulation of wave and particle transport in various media is the key driving force for modern information processing and communication. In a strongly scattering medium, waves and particles exhibit versatile transport characteristics such as localization, tunnelling with exponential decay, ballistic, and diffusion behaviours due to dynamical multiple scattering from strong scatters or impurities. Recent investigations of graphene have offered a unique approach, from a quantum point of view, to design the dispersion of electrons on demand, enabling relativistic massless Dirac quasiparticles, and thus inducing low-loss transport either ballistically or diffusively. Here, we report an experimental demonstration of an artificial phononic graphene tailored for surface phonons on a LiNbO3 integrated platform. The system exhibits Dirac quasiparticle-like transport, that is, pseudo-diffusion at the Dirac point, which gives rise to a thickness-independent temporal beating for transmitted pulses, an analogue of Zitterbewegung effects. The demonstrated fully integrated artificial phononic graphene platform here constitutes a step towards on-chip quantum simulators of graphene and unique monolithic electro-acoustic integrated circuits.
Sub-Poissonian phonon statistics in an acoustical resonator coupled to a pumped two-level emitter
Energy Technology Data Exchange (ETDEWEB)
Ceban, V., E-mail: victor.ceban@phys.asm.md; Macovei, M. A., E-mail: macovei@phys.asm.md [Academy of Sciences of Moldova, Institute of Applied Physics (Moldova, Republic of)
2015-11-15
The concept of an acoustical analog of the optical laser has been developed recently in both theoretical and experimental works. We here discuss a model of a coherent phonon generator with a direct signature of the quantum properties of sound vibrations. The considered setup is made of a laser-driven quantum dot embedded in an acoustical nanocavity. The system dynamics is solved for a single phonon mode in the steady-state and in the strong quantum dot—phonon coupling regime beyond the secular approximation. We demonstrate that the phonon statistics exhibits quantum features, i.e., is sub-Poissonian.
Electron-phonon coupling in hybrid lead halide perovskites.
Wright, Adam D; Verdi, Carla; Milot, Rebecca L; Eperon, Giles E; Pérez-Osorio, Miguel A; Snaith, Henry J; Giustino, Feliciano; Johnston, Michael B; Herz, Laura M
2016-05-26
Phonon scattering limits charge-carrier mobilities and governs emission line broadening in hybrid metal halide perovskites. Establishing how charge carriers interact with phonons in these materials is therefore essential for the development of high-efficiency perovskite photovoltaics and low-cost lasers. Here we investigate the temperature dependence of emission line broadening in the four commonly studied formamidinium and methylammonium perovskites, HC(NH2)2PbI3, HC(NH2)2PbBr3, CH3NH3PbI3 and CH3NH3PbBr3, and discover that scattering from longitudinal optical phonons via the Fröhlich interaction is the dominant source of electron-phonon coupling near room temperature, with scattering off acoustic phonons negligible. We determine energies for the interacting longitudinal optical phonon modes to be 11.5 and 15.3 meV, and Fröhlich coupling constants of ∼40 and 60 meV for the lead iodide and bromide perovskites, respectively. Our findings correlate well with first-principles calculations based on many-body perturbation theory, which underlines the suitability of an electronic band-structure picture for describing charge carriers in hybrid perovskites.
Electron-phonon coupling in hybrid lead halide perovskites
Wright, Adam D.; Verdi, Carla; Milot, Rebecca L.; Eperon, Giles E.; Pérez-Osorio, Miguel A.; Snaith, Henry J.; Giustino, Feliciano; Johnston, Michael B.; Herz, Laura M.
2016-05-01
Phonon scattering limits charge-carrier mobilities and governs emission line broadening in hybrid metal halide perovskites. Establishing how charge carriers interact with phonons in these materials is therefore essential for the development of high-efficiency perovskite photovoltaics and low-cost lasers. Here we investigate the temperature dependence of emission line broadening in the four commonly studied formamidinium and methylammonium perovskites, HC(NH2)2PbI3, HC(NH2)2PbBr3, CH3NH3PbI3 and CH3NH3PbBr3, and discover that scattering from longitudinal optical phonons via the Fröhlich interaction is the dominant source of electron-phonon coupling near room temperature, with scattering off acoustic phonons negligible. We determine energies for the interacting longitudinal optical phonon modes to be 11.5 and 15.3 meV, and Fröhlich coupling constants of ~40 and 60 meV for the lead iodide and bromide perovskites, respectively. Our findings correlate well with first-principles calculations based on many-body perturbation theory, which underlines the suitability of an electronic band-structure picture for describing charge carriers in hybrid perovskites.
Makovetskii, D N
2012-01-01
A problem of self-organized motions in solid-state nonequilibrium media has been studied experimentally using methods of quantum acoustics. Generalized Poincare cross-sections of microwave power spectra (MPS) have been obtained in an optical-wavelengths acoustic laser (paramagnetic phaser) based on ruby crystal. Considerable narrowing of MPS and their autowave-like superslow motion have been observed under conditions of periodical pump modulation beyond the region of the phaser relaxation resonance. Some preliminar experimental results of this work were published in: Solid State Communications, Vol.90, No.8, P.501 (1994). An interpretation of the experimental data see arXiv:1101.0482v1 ; arXiv:cond-mat/0410460v1 ; arXiv:cond-mat/0303188v1 .
Laser action at 16. mu. by optical pumping of CO/sub 2/ with an HF laser
Energy Technology Data Exchange (ETDEWEB)
Kuntsevich, B.F.; Stepanov, B.I.; Trushin, S.A.; Churakov, V.V.
1977-08-01
Calculations are presented on the threshold properties of a CO/sub 2/ laser that is optically pumped by the P/sub 1/(7) line of a HF laser. The dependence on the CO/sub 2/ pressure is considered.(AIP)
Tunable Topological Phononic Crystals
Chen, Ze-Guo
2016-05-27
Topological insulators first observed in electronic systems have inspired many analogues in photonic and phononic crystals in which remarkable one-way propagation edge states are supported by topologically nontrivial band gaps. Such band gaps can be achieved by breaking the time-reversal symmetry to lift the degeneracy associated with Dirac cones at the corners of the Brillouin zone. Here, we report on our construction of a phononic crystal exhibiting a Dirac-like cone in the Brillouin zone center. We demonstrate that simultaneously breaking the time-reversal symmetry and altering the geometric size of the unit cell result in a topological transition that we verify by the Chern number calculation and edge-mode analysis. We develop a complete model based on the tight binding to uncover the physical mechanisms of the topological transition. Both the model and numerical simulations show that the topology of the band gap is tunable by varying both the velocity field and the geometric size; such tunability may dramatically enrich the design and use of acoustic topological insulators.
Kamaraju, N.; Kumar, Sunil; Anija, M.; Sood, A. K.
2010-11-01
We report femtosecond time-resolved reflectivity measurements of coherent phonons in tellurium performed over a wide range of temperatures (3-296 K) and pump-laser intensities. A totally symmetric A1 coherent phonon at 3.6 THz responsible for the oscillations in the reflectivity data is observed to be strongly positively chirped (i.e., phonon time period decreases at longer pump-probe delay times) with increasing photoexcited carrier density, more so at lower temperatures. We show that the temperature dependence of the coherent phonon frequency is anomalous (i.e, increasing with increasing temperature) at high photoexcited carrier density due to electron-phonon interaction. At the highest photoexcited carrier density of ˜1.4×1021cm-3 and the sample temperature of 3 K, the lattice displacement of the coherent phonon mode is estimated to be as high as ˜0.24Å . Numerical simulations based on coupled effects of optical absorption and carrier diffusion reveal that the diffusion of carriers dominates the nonoscillatory electronic part of the time-resolved reflectivity. Finally, using the pump-probe experiments at low carrier density of 6×1018cm-3 , we separate the phonon anharmonicity to obtain the electron-phonon coupling contribution to the phonon frequency and linewidth.
Photo-excited charge carriers suppress sub-terahertz phonon mode in silicon at room temperature
Liao, Bolin; Maznev, A. A.; Nelson, Keith A.; Chen, Gang
2016-01-01
There is a growing interest in the mode-by-mode understanding of electron and phonon transport for improving energy conversion technologies, such as thermoelectrics and photovoltaics. Whereas remarkable progress has been made in probing phonon–phonon interactions, it has been a challenge to directly measure electron–phonon interactions at the single-mode level, especially their effect on phonon transport above cryogenic temperatures. Here we use three-pulse photoacoustic spectroscopy to investigate the damping of a single sub-terahertz coherent phonon mode by free charge carriers in silicon at room temperature. Building on conventional pump–probe photoacoustic spectroscopy, we introduce an additional laser pulse to optically generate charge carriers, and carefully design temporal sequence of the three pulses to unambiguously quantify the scattering rate of a single-phonon mode due to the electron–phonon interaction. Our results confirm predictions from first-principles simulations and indicate the importance of the often-neglected effect of electron–phonon interaction on phonon transport in doped semiconductors. PMID:27731406
Yu, Chung; Chong, Yat C.; Fong, Chee K.
1989-06-01
Interaction of GHz and MHz radiation with CO2 laser propagation in a silver halide fiber using sBs based phonon coupling is furthet investigated. The external signal serves to both probe and enhance laser generated sBs phonons in the fiber. Efficient coupling of microwave radiation into the fiber is accomplished by placing the fiber in a hollow metallic waveguide, designed and constructed to transmit the dominant mode in the 0.9-2.0 GHz band. MHz radiation is conveniently coupled into the fiber using the guided microwave radiation as carrier. Phonon emissions from the fiber under CO2 laser pumping are first established on a spectrum analyzer; low frequency generators ale then tuned to match these frequencies and their maximum interaction recorded. Such interactions are systematically studied by monitoring the amplitude and waveform of the reflected and transmitted laser pulse at various power levels and frequencies of the externally coupled radiation. A plot of reflected laser power versus incident laser power reveals a distinct sBs generated phonon threshold. Variouslaunch directions of the GHz and MHz radiation with respect to the direction of laser propagation are realized to verify theory governing sBs interactions. The MHz radiation and its associated phonons in the fiber are convenient tools for probing sBs related phenomenon in infrared fibers.
Annenkov, Vadim V; Kozlov, Alexander S; Danilovtseva, Elena N; Basharina, Tatjana N; Petrov, Alexander K
2013-07-01
Diatom algae realize highly intriguing processes of biosynthesis of siliceous structures in living cells under moderate conditions. Investigation of diatom physiology is complicated by frustule (siliceous exoskeleton). Frustules consist of valves and girdle bands which are adhered to each other by means of organic substances. Removal of the frustule from the lipid membrane of diatom cells would open new possibilities for study of silicon metabolism in diatoms. We found that submillimeter laser irradiation produced by a free-electron laser causes splitting of diatom frustules without destruction of cell content. This finding opens the way to direct study of diatom cell membrane and to isolation of cell organelles, including silica deposition vesicles. We suppose that the dissection action of the submillimeter irradiation results from unusual ultrasonic waves produced by the short (30-100 ps) but high-power (1 MW) terahertz laser impulses at 5.6 MHz frequency.
Energy Technology Data Exchange (ETDEWEB)
Osychenko, A A; Zalesskii, A D; Krivokharchenko, A S; Zhakhbazyan, A K; Nadtochenko, V A [N N Semenov Institute of Chemical Physics, Russian Academy of Sciences, Moscow (Russian Federation); Ryabova, A V [A M Prokhorov General Physics Institute, Russian Academy of Sciences, Moscow (Russian Federation)
2015-05-31
Using the method of femtosecond laser surgery we study the fusion of two-cell mouse embryos under the action of tightly focused femtosecond laser radiation with the fusion efficiency reaching 60%. The detailed statistical analysis of the efficiency of blastomere fusion and development of the embryo up to the blastocyst stage after exposure of the embryos from different mice to a femtosecond pulse is presented. It is shown that the efficiency of blastocyst formation essentially depends on the biological characteristics of the embryo, namely, the strain and age of the donor mouse. The possibility of obtaining hexaploid embryonal cells using the methods of femtosecond laser surgery is demonstrated. (extreme light fields and their applications)
Ruby laser-assisted depilation: The mode of action and potential ways of improved outcome
Topping, Adam Partington
Aim - To improve efficacy and lessen side effects resulting from normal mode ruby laser (NMRL)-assisted depilation via a greater understanding of its mode of action and the development of novel methods of reducing associated epidermal damage. Employing a thermal imaging camera and ex vivo hair-bearing skin, the targets for the NMRL (pulse duration 900 musec and spot size 7 mm) were defined, the temperatures reached and the heat dissipation rates determined. Production of heat was confined to the hair follicles, with the peak temperatures reached varying considerably between hairs within the same treatment area and also between individuals. Histological assessment for a known indicator of cellular damage (p53 expression) identified the sites and extent of damage, which correlated with the peak temperatures measured. An energy meter was used to detect the penetration of NMRL light through ex vivo skin, which was found to be deeper than previously theorised. The black-haired mouse (C57B1/10) was assessed both macroscopically and histologically and found to be an acceptable animal model of NMRL depilation and associated epidermal damage. Attempts to reduce the epidermal damage by simply stopping the light reaching the epidermis using a chromophore block were assessed. Chromophore did indeed reduce the amount of epidermal damage detected in laser-irradiated ex vivo human skin, whereas in contrast it increased the wounding seen in the much thinner skin of the mouse. Nevertheless the mouse model showed that this technique did not affect the depilation efficacy. An alternative method of reducing epidermal damage using induction of the cells' intrinsic protective mechanisms (heat shock proteins, HSP) was assessed using cultured keratinocytes and the mouse model. Primarily, the sub-lethal temperature optimum for HSP expression in human keratinocytes was determined, then an in vitro model of NMRL-associated epidermal damage was established and the heat pre-treatment assessed
Wong, Joe
2004-03-01
The phonon spectra of plutonium and its alloys have been sought after in the past few decades following the discovery of this actinide element in 1941, but with no success. This was due to a combination of the high neutron absorption cross section of 239Pu, the common isotope, and non-availability of large single crystals of any Pu-bearing materials. We have recent designed a high resolution inelastic x-ray scattering experiment using a bright synchrotron x-ray beam at the European Sychrotron Radiation Facility (ESRF), Grenoble and mapped the full phonon dispersion curves of an fcc delta-phase polycrystalline Pu-Ga alloy (1). Several unusual features including, a large elastic anisotropy, a small shear elastic modulus C', a Kohn-like anomaly in the T1[011] branch, and a pronounced softening of the [111] transverse modes are found. These features can be related to the phase transitions of plutonium and to strong coupling between the lattice structure and the 5f valence instabilities. Our results also provide a critical test for theoretical treatments of highly correlated 5f electron systems as exemplified by recent dynamical mean field theory (DMFT) calculations for d-plutonium.(2) This work was performed in collaboration with Dr. M. Krisch (ESRF)) and Prof. T.-C. Chiang (UIU), and under the auspices of the U. S. Department of Energy by the University of California, Lawrence Livermore National Laboratory under Contract No. W-7405-Eng-48. 1. Joe Wong et al. Science, vol.301, 1078 (2003) 2. X. Dai et al. Science, vol.300, 953 (2003)
Gravitational Perturbation in Topological Phonon Space
Institute of Scientific and Technical Information of China (English)
李芳昱; 罗俊; 唐孟希
1994-01-01
The effect of gravitational wave (GW) on phonon in crystal lattice space with spiral dislocation is expressed as a gravitational perturbation in topological phonon space with background of the spiral dislocation.This is a new-type effect form of the GW field to the phonon.The corresponding phonon solutions are given.
Piezoelectric surface acoustical phonon amplification in graphene on a GaAs substrate
Nunes, O. A. C.
2014-06-01
We study the interaction of Dirac Fermions in monolayer graphene on a GaAs substrate in an applied electric field by the combined action of the extrinsic potential of piezoelectric surface acoustical phonons of GaAs (piezoelectric acoustical (PA)) and of the intrinsic deformation potential of acoustical phonons in graphene (deformation acoustical (DA)). We find that provided the dc field exceeds a threshold value, emission of piezoelectric (PA) and deformation (DA) acoustical phonons can be obtained in a wide frequency range up to terahertz at low and high temperatures. We found that the phonon amplification rate RPA ,DA scales with TBGS -1 (S =PA,DA), TBGS being the Block -Gru¨neisen temperature. In the high-T Block -Gru¨neisen regime, extrinsic PA phonon scattering is suppressed by intrinsic DA phonon scattering, where the ratio RPA/RDA scales with ≈1/√n , n being the carrier concentration. We found that only for carrier concentration n ≤1010cm-2, RPA/RDA>1. In the low-T Block -Gru¨neisen regime, and for n =1010cm-2, the ratio RPA/RDA scales with TBGDA/TBGPA≈7.5 and RPA/RDA>1. In this regime, PA phonon dominates the electron scattering and RPA/RDA<1 otherwise. This study is relevant to the exploration of the acoustic properties of graphene and to the application of graphene as an acoustical phonon amplifier and a frequency-tunable acoustical phonon device.
Phonon-drag effects on thermoelectric power
Wu, M. W.; Horing, N. J. M.; Cui, H. L.
1995-01-01
We carry out a calculation of the phonon-drag contribution $S_g$ to the thermoelectric power of bulk semiconductors and quantum well structures for the first time using the balance equation transport theory extended to the weakly nonuniform systems. Introducing wavevector and phonon-mode dependent relaxation times due to phonon-phonon interactions, the formula obtained can be used not only at low temperatures where the phonon mean free path is determined by boundary scattering, but also at hi...
Yin, Jiajia; Feng, Guoying; Zhou, Shouhuan; Zhang, Hong; Wang, Shutong; Zhang, Hua
2016-10-01
Random laser actions in a disordered media based on polymethyl methacrylate (PMMA) polymer doped with Rh6G dye and Au nanoparticles have been demonstrated. It was observed that the shape of Au nanoparticles can tune the spectral central position of the random laser action. It was also seen that the shape of Au nanoparticles strongly affects the pump threshold. Comparing nanosphere- and nanorod-based systems, the nanorod-based one exhibited a lower threshold.
Anomalous effect of phonon wind on lateral migration of excitons in ultrathin quantum CdTe/ZnTe well
Onishchenko, E E; Zajtsev, V V
2001-01-01
The effect of the acoustic phonons nonequilibrium flux on the photoluminescence of the CdTe/ZnTe thin quantum well, excited quasi-resonantly by the He-Ne-laser is studied. It is established that the phonon flux leads to the change in the form of the quantum well luminescence band even by low generation capacities. It is assumed that the nonequilibrium phonons flux stimulates the excitons migration in the quantum well plane, conditioned by the tunnel transitions between the potential local minima, which are accompanied by the phonons induced emission
Photonic and phononic quasicrystals
Energy Technology Data Exchange (ETDEWEB)
Steurer, Walter; Sutter-Widmer, Daniel [Laboratory of Crystallography, Department of Materials, ETH Zurich, Wolfgang-Pauli-Strasse 10, CH-8093 Zurich (Switzerland)
2007-07-07
This review focuses on the peculiarities of quasiperiodic order for the properties of photonic and phononic (sonic) heterostructures. The most beneficial feature of quasiperiodicity is that it can combine perfectly ordered structures with purely point-diffractive spectra of arbitrarily high rotational symmetry. Both are prerequisites for the construction of isotropic band gap composites, in particular from materials with low index contrast, which are required for numerous applications. Another interesting property of quasiperiodic structures is their scaling symmetry, which may be exploited to create spectral gaps in the sub-wavelength regime. This review covers structure/property relationships of heterostructures based on one-dimensional (1D) substitutional sequences such as the Fibonacci, Thue-Morse, period-doubling, Rudin-Shapiro and Cantor sequence as well as on 1D modulated structures, further on 2D tilings with 8-, 10-, 12- and 14-fold symmetry as well as on the pinwheel tiling, the Sierpinski gasket and on curvilinear tilings and, finally, on the 3D icosahedral Penrose tiling. (topical review)
Isotope Effect on Electron-Phonon Coupling in Multiband Superconductor MgB2
Mou, Daixiang; Taufour, Valentin; Wu, Yun; Huang, Lunan; Bud'Ko, Serguei; Canfield, Paul; Kaminski, Adam
We systematically investigate the isotope effect of electron-phonon coupling in multi-band superconductor MgB2 by laser based Angle Resolved Photoemission Spectroscopy. The kink structure around 70 meV on two σ bands, which is caused by electron coupling to E2 g phonon mode, is shifted to higher binding energy in Mg10B2 than that in Mg11B2. The measured shifting energy of 3.5 meV is consistent with theoretical calculation based on harmonic phonon in MgB2. Our temperature dependent measurement also indicates the isotope effect of kink structure is not dependent on superconducting transition.
Dephasing times in quantum dots due to elastic LO phonon-carrier collisions
DEFF Research Database (Denmark)
Uskov, A. V.; Jauho, Antti-Pekka; Tromborg, Bjarne;
2000-01-01
Interpretation of experiments on quantum dot (QD) lasers presents a challenge: the phonon bottleneck, which should strongly suppress relaxation and dephasing of the discrete energy states, often seems to be inoperative. We suggest and develop a theory for an intrinsic mechanism for dephasing in QDs......: second-order elastic interaction between quantum dot charge carriers and LO phonons. The calculated dephasing times are of the order of 200 fs at room temperature, consistent with experiments. The phonon bottleneck thus does not prevent significant room temperature dephasing....
Coherent phonons in carbon nanotubes and graphene
Kim, J.-H.; Nugraha, A. R. T.; Booshehri, L. G.; Hároz, E. H.; Sato, K.; Sanders, G. D.; Yee, K.-J.; Lim, Y.-S.; Stanton, C. J.; Saito, R.; Kono, J.
2013-02-01
We review recent studies of coherent phonons (CPs) corresponding to the radial breathing mode (RBM) and G-mode in single-wall carbon nanotubes (SWCNTs) and graphene. Because of the bandgap-diameter relationship, RBM-CPs cause bandgap oscillations in SWCNTs, modulating interband transitions at terahertz frequencies. Interband resonances enhance CP signals, allowing for chirality determination. Using pulse shaping, one can selectively excite specific-chirality SWCNTs within an ensemble. G-mode CPs exhibit temperature-dependent dephasing via interaction with RBM phonons. Our microscopic theory derives a driven oscillator equation with a density-dependent driving term, which correctly predicts CP trends within and between (2n + m) families. We also find that the diameter can initially increase or decrease. Finally, we theoretically study the radial breathing like mode in graphene nanoribbons. For excitation near the absorption edge, the driving term is much larger for zigzag nanoribbons. We also explain how the armchair nanoribbon width changes in response to laser excitation.
Phononics in low-dimensional materials
Directory of Open Access Journals (Sweden)
Alexander A. Balandin
2012-06-01
Full Text Available Phonons – quanta of crystal lattice vibrations – reveal themselves in all electrical, thermal, and optical phenomena in materials. Nanostructures open exciting opportunities for tuning the phonon energy spectrum and related material properties for specific applications. The possibilities for controlled modification of the phonon interactions and transport – referred to as phonon engineering or phononics – increased even further with the advent of graphene and two-dimensional van der Waals materials. We describe methods for tuning the phonon spectrum and engineering the thermal properties of the low-dimensional materials via ribbon edges, grain boundaries, isotope composition, defect concentration, and atomic-plane orientation.
Sideband Raman Cooling of Optical Phonons in Semiconductors
Zhang, Jun; Kwek, Leong Chuan; Xiong, Qihua
2014-03-01
Last century has witnessed a tremendous success of laser cooling technology from trapped atomic ions to solid-state optical refrigeration. As one of the laser cooling techniques, sideband Raman cooling plays an important role in quantum ground state preparation, coherent quantum-state manipulation and quantum phenomena study. However, those studies still limited in trapped atomic ions and cavity optomechanics, which need be cooled it below than 0.1 Kelvin even tens of nano-Kelvin due to very low frequency of phonons from several kHz to GHz. Here we report sideband Raman cooling and heating experiments of longitudinal optical phonon (LOP) with a 6.23 THz in semiconductor ZnTe nano-ribbons. By using of red-sideband laser, we cool the LOP from 225 to 55 Kelvin, corresponding to an average occupation number reduced from 0.36 to 0.005. We also observe a LOPs heating from 230 to 384 Kelvin with a blue-sideband pumping. Our experiment opens a possibility of all solid state quantum applications using semiconductor optical phonon mediated coupling at room temperature. We gratefully acknowledge funding from Singapore NRF, MOE and NTU.
Electron-Phonon Coupling and Energy Flow in a Simple Metal beyond the Two-Temperature Approximation
Waldecker, Lutz; Bertoni, Roman; Ernstorfer, Ralph; Vorberger, Jan
2016-04-01
The electron-phonon coupling and the corresponding energy exchange are investigated experimentally and by ab initio theory in nonequilibrium states of the free-electron metal aluminium. The temporal evolution of the atomic mean-squared displacement in laser-excited thin freestanding films is monitored by femtosecond electron diffraction. The electron-phonon coupling strength is obtained for a range of electronic and lattice temperatures from density functional theory molecular dynamics simulations. The electron-phonon coupling parameter extracted from the experimental data in the framework of a two-temperature model (TTM) deviates significantly from the ab initio values. We introduce a nonthermal lattice model (NLM) for describing nonthermal phonon distributions as a sum of thermal distributions of the three phonon branches. The contributions of individual phonon branches to the electron-phonon coupling are considered independently and found to be dominated by longitudinal acoustic phonons. Using all material parameters from first-principles calculations except the phonon-phonon coupling strength, the prediction of the energy transfer from electrons to phonons by the NLM is in excellent agreement with time-resolved diffraction data. Our results suggest that the TTM is insufficient for describing the microscopic energy flow even for simple metals like aluminium and that the determination of the electron-phonon coupling constant from time-resolved experiments by means of the TTM leads to incorrect values. In contrast, the NLM describing transient phonon populations by three parameters appears to be a sufficient model for quantitatively describing electron-lattice equilibration in aluminium. We discuss the general applicability of the NLM and provide a criterion for the suitability of the two-temperature approximation for other metals.
Phonon spectra in quantum wires
Directory of Open Access Journals (Sweden)
Ilić Dušan
2007-01-01
Full Text Available Green's function method, adjusted to bound crystalline structures, was applied to obtain the phonon dispersion law in quantum wires. The condition of the existence of small mechanical atom movements defining phonon spectra can be found by solving the secular equation. This problem was presented graphically for different boundary parameters. The presence of boundaries, as well as the change of boundary parameters, leads to the appearance of new properties of the layered structure. The most important feature is that, beside the allowed energy zones (which are continuous as in the bulk structure, zones of forbidden states appear. Different values of the boundary parameters lead to the appearance of lower and upper energy gaps, or dispersion branches spreading out of the bulk energy zone. The spectra of phonons in corresponding unbound structures were correlated to those in bound structures.
Phonon creation by gravitational waves
Sabín, Carlos; Ahmadi, Mehdi; Fuentes, Ivette
2014-01-01
We show that gravitational waves create phonons in a Bose-Einstein condensate (BEC). A traveling spacetime distortion produces particle creation resonances that correspond to the dynamical Casimir effect in a BEC phononic field contained in a cavity-type trap. We propose to use this effect to detect gravitational waves. The amplitude of the wave can be estimated applying recently developed relativistic quantum metrology techniques. We provide the optimal precision bound on the estimation of the wave's amplitude. Finally, we show that the parameter regime required to detect gravitational waves with this technique is within experimental reach.
Selective coherent phonon mode generation in single wall carbon nanotubes
Nugraha, Ahmad R T; Saito, Riichiro
2016-01-01
The ultrafast pulse-train technique is theoretically investigated to enhance a specific coherent phonon mode while suppressing the other phonon modes generated in single wall carbon nanotubes (SWNTs). In particular, we focus on the selectivity of the radial breathing mode (RBM) and the G-band for a given SWNT. We find that if the repetition period matches with integer multiple of the RBM phonon period, the RBM amplitude could be enhanced while the amplitudes of the other modes are suppressed. As for the G-band, when we apply a repetition rate of half-integer multiple of the RBM period, the RBM could be suppressed because of destructive interference, while the G-band still survives. It is also possible to keep the G-band and suppress the RBM by applying a repetition rate that matches with integer multiple of the G-band phonon period. However, in this case we have to use a large number of laser pulses.
Action of a 904-nm diode laser in orthopedics and traumatology: a clinical study on 447 cases
Tam, Giuseppe
2001-10-01
Objective: The evidence in medical literature is that a beneficial analgesic effect can only be obtained by employing laser radiation of relatively low power density and wavelengths which are able to penetrate tissue. For this reason the semiconductor, or laser diode (GaAs, 904 nm), is the most appropriate choice in pain-reduction therapy. Summary Background Data: Low power laser (or LLL) acts on the Prostaglandins synthesis, increases the endorphins synthesis in the Rolando gelatinous substance and in the dorsal horn of the spinal cord. The L-Arginine, which is the classic substrate of nitric oxide, carries on vasodilatory and anti- inflammatory action. Methods: Treatment was carried out on 447 cases and 435 patients (250 women and 185 men) between 20th May 1987 and 31st December 1999. The patients, whose age ranged from 25 to 70, were suffering from rheumatic, degenerative and traumatic pathologies as well as cutaneous ulcers. The majority of patients had been seen by orthopaedists and rheumatologists and had undergone x-ray, ultrasound scan, etc. All patients had previously received drug-based treatment and/or physiotherapy, with poor results. Two thirds were experiencing acute symptomatic pain, while the others presented a chronic pathology with recurrent crises. We used a pulsed IR diode laser, GaAs emitting at 904 nm. Frequency of treatment: 1 application per day for 5 consecutive days, followed by a 2-day interval. The percentage reduction in symptoms or improvement in functional status were determined on the basis of objective analysis as it happens in the Legal and Insurance Medicine field. Results: Very good results were achieved especially with cases of symptomatic osteoarthritis of the cervical vertebrae, with sport-related injuries, epicondylitis, osteoarthritis of the knee, periarthritis and with cutaneous ulcers. The beneficial action of the LLLT in the latter pathology is linked to the increase in collagen and to fibroblast proliferation. The total
Structure of the phonon vacuum state
Mishev, S
2012-01-01
The action of the long-range residual force on the the expectation value of observables in the nuclear ground-states is evaluated by finding optimal values for the coefficients of the canonical transformation which connects the phonon vacuum state with the (quasi-)particle ground-state. After estimating the improvements over the predictions of the independent particle approximation we compare the ground-state wave functions obtained using the presented approach with those obtained using the conventional random phase approximation (RPA) and its extended version. The problem with overbinding of the nuclear ground state calculated using the RPA is shown to be removed if one sticks to the prescriptions of the present approach. The reason being that the latter conforms to the original variational formulation. Calculations are performed within the two-level Lipkin model in which we present results for the binding energies.
The heat-pipe resembling action of boiling bubbles in endovenous laser ablation
C.W.M. van der Geld (Cees); R.R. van den Bos (Renate); P.W.M. van Ruijven (Peter); T.E.C. Nijsten (Tamar); H.A.M. Neumann (Martino); M.J.C. van Gemert (Martin)
2010-01-01
textabstractEndovenous laser ablation (EVLA) produces boiling bubbles emerging from pores within the hot fiber tip and traveling over a distal length of about 20 mm before condensing. This evaporation-condensation mechanism makes the vein act like a heat pipe, where very efficient heat transport mai
The heat-pipe resembling action of boiling bubbles in endovenous laser ablation
van der Geld, C.W.M.; van den Bos, R.R.; van Ruijven, P.W.M.; Nijsten, T.; Neumann, H.A.M.; van Gemert, M.J.C.
2010-01-01
Endovenous laser ablation (EVLA) produces boiling bubbles emerging from pores within the hot fiber tip and traveling over a distal length of about 20 mm before condensing. This evaporation-condensation mechanism makes the vein act like a heat pipe, where very efficient heat transport maintains a con
EMRS Spring Meeting 2014 Symposium D: Phonons and fluctuations in low dimensional structures
2014-11-01
. Goettingen) poster title ''Phonon blocking in Multilayers produced by Pulsed Laser Deposition'', Jordi Gomis-Bresco et al. (ICN2) poster '' A 1D PhoXonic Crystal'', Barcelona and Benjamin J Robinson et al. (U. Lancaster) poster ''Scanning Thermal microscopy studies of 2D materials''. The symposium organisers are grateful to the Scientific Committee members, Prof. Bahram Djafari-Rouhani (France), Prof. Dr. Thomas Dekorsy (Germany), Prof. Anthony Kent (UK), Prof. Fabio Marchesoni (Italy), Dr. Natalio Mingo (France), Prof. Pascal Ruello, (France) and Prof. Javier Viejo-Rodriguez (Spain), for their help with all aspects of evaluation of the scientific level of the presentations in the symposium. The symposium was sponsored by the FP7 ICT FET Open Coordination Action EUPHONON (GA. 612086) and by the CNRS GDR ''Thermal Nanosciences and NanoEngineering''. The symposium organisers express their sincere thanks to the staff of the E-MRS for continuous support and timely advice in all organisational aspects. We are indebted to Dr. Erwan Guillotel (ICN2) for his assistance with the organisation of the symposium.
Energy Technology Data Exchange (ETDEWEB)
Otelaja, O. O. [School of Electrical and Computer Engineering, Cornell University, Ithaca, New York 14853 (United States); Robinson, R. D., E-mail: rdr82@cornell.edu [Department of Materials Science and Engineering, Cornell University, Ithaca, New York 14853 (United States)
2015-10-26
In this work, the mechanism for enhanced phonon backscattering in silicon is investigated. An understanding of phonon propagation through substrates has implications for engineering heat flow at the nanoscale, for understanding sources of decoherence in quantum systems, and for realizing efficient phonon-mediated particle detectors. In these systems, phonons that backscatter from the bottom of substrates, within the crystal or from interfaces, often contribute to the overall detector signal. We utilize a microscale phonon spectrometer, comprising superconducting tunnel junction emitters and detectors, to specifically probe phonon backscattering in silicon substrates (∼500 μm thick). By etching phonon “enhancers” or deep trenches (∼90 μm) around the detectors, we show that the backscattered signal level increases by a factor of ∼2 for two enhancers versus one enhancer. Using a geometric analysis of the phonon pathways, we show that the mechanism of the backscattered phonon enhancement is due to confinement of the ballistic phonon pathways and increased scattering off the enhancer walls. Our result is applicable to the geometric design and patterning of substrates that are employed in phonon-mediated detection devices.
Nonlinear phononics using atomically thin membranes
Midtvedt, Daniel; Isacsson, Andreas; Croy, Alexander
2014-09-01
Phononic crystals and acoustic metamaterials are used to tailor phonon and sound propagation properties by utilizing artificial, periodic structures. Analogous to photonic crystals, phononic band gaps can be created, which influence wave propagation and, more generally, allow engineering of the acoustic properties of a system. Beyond that, nonlinear phenomena in periodic structures have been extensively studied in photonic crystals and atomic Bose-Einstein condensates in optical lattices. However, creating nonlinear phononic crystals or nonlinear acoustic metamaterials remains challenging and only few examples have been demonstrated. Here, we show that atomically thin and periodically pinned membranes support coupled localized modes with nonlinear dynamics. The proposed system provides a platform for investigating nonlinear phononics.
Magnon-phonon interconversion in a dynamically reconfigurable magnetic material
Guerreiro, Sergio C.; Rezende, Sergio M.
2015-12-01
The ferrimagnetic insulator yttrium iron garnet (YIG) is an important material in the field of magnon spintronics, mainly because of its low magnetic losses. YIG also has very low acoustic losses, and for this reason the conversion of a state of magnetic excitation (magnons) into a state of lattice vibration (phonons), or vice versa, broadens its possible applications in spintronics. Since the magnetic parameters can be varied by some external action, the magnon-phonon interconversion can be tuned to perform a desired function. We present a quantum theory of the interaction between magnons and phonons in a ferromagnetic material subject to a dynamic variation of the applied magnetic field. It is shown that when the field gradient at the magnetoelastic crossover region is much smaller than a critical value, an initial elastic excitation can be completely converted into a magnetic excitation, or vice versa. This occurs with conservation of linear momentum and spin angular momentum, implying that phonons created by the conversion of magnons have spin angular momentum and carry spin current. It is shown further that if the system is initially in a quantum coherent state, its coherence properties are maintained regardless of the time dependence of the field.
Ab initio calculations of phonon dispersion and lattice dynamics in TlGaTe{sub 2}
Energy Technology Data Exchange (ETDEWEB)
Jafarova, Vusala; Orudzhev, Guseyn; Alekperov, Oktay; Mamedov, Nazim; Abdullayev, Nadir; Najafov, Arzu [Institute of Physics (Innovation Sector), 33 H. Javid ave, Baku 1143 (Azerbaijan); Paucar, Raul [Institute of Physics (Innovation Sector), 33 H. Javid ave, Baku 1143 (Azerbaijan); Chiba Institute of Technology, 2-17-1 Tsudanuma, Narashino, Chiba 275-0016 (Japan); Shim, YongGu [Osaka Prefecture University, 1-1 Gakuen-cho, Naka-ku, Sakai, Osaka 599-8531 (Japan); Wakita, Kazuki [Chiba Institute of Technology, 2-17-1 Tsudanuma, Narashino, Chiba 275-0016 (Japan)
2015-06-15
This work reports the results of DFT-based calculations of phonon spectra of TlGaTe{sub 2}. The dispersion of phonon bands was calculated along the directions of Brillouin zone (BZ) that include symmetry points. The calculated phonon frequencies at the centre of BZ were compared with those obtained by Raman spectroscopy with the aid of a confocal laser microscopy system. A fairly good agreement between the calculated and experimental data was found. Complimentary, molar heat capacity at constant volume and Debye temperature were calculated in the range 5/500 K on the base of the obtained phonon density of states. The obtained temperature dependencies were compared with available experimental data.The results of comparison were satisfactory. (copyright 2015 WILEY-VCH Verlag GmbH and Co. KGaA, Weinheim)
Golubev, V B
2001-01-01
The hydrodynamic model of the periodical lamination of the heterogeneous condensed systems from the immiscible components under the effect of the powerful laser beams in the mode of canalized permittivity is presented. The model accounts for the motion of the immiscible components particles in the melt vortex flows under the effect of the centrifugal forces. The conditions for origination of the periodical concentration lamination and their spatial scale are determined
Theory of coherent phonons in graphene
Sanders, G. D.; Stanton, C. J.; Kim, J.-H.; Yee, K.-J.; Jung, M. H.; Hong, B. H.; Haroz, E. H.; Kono, J.
2011-03-01
We develop a theory for the generation and detection of coherent phonons in graphene. Coherent phonons are generated via the deformation potential electron-phonon interaction with photogenerated carriers. In our theory the electronic states are treated in a third nearest neighbor extended tight binding formalism which gives a good description of the states over the entire graphene Brillouin zone while the phonon states are treated in a valence force field model. The equations of motion for the coherent phonon amplitudes are obtained in a density matrix formalism and we find that the coherent phonon amplitudes satisfy driven oscillator equations for each value of the phonon wavevector. Comparison is made with recent experimental measurements. Supported by NSF through grants OISE-0530220 and DMR-0706313 and the ONR through grant ONR-00075094, and the Robert A. Welch Foundation through grant No. C-1509.
A holographic perspective on phonons and pseudo-phonons
Amoretti, Andrea; Argurio, Riccardo; Musso, Daniele; Zayas, Leopoldo A Pando
2016-01-01
We analyze the concomitant spontaneous breaking of translation and conformal symmetries by introducing in a CFT a complex scalar operator that acquires a spatially dependent expectation value. The model, inspired by the holographic Q-lattice, provides a privileged setup to study the emergence of phonons from a spontaneous translational symmetry breaking in a conformal field theory and offers valuable hints for the treatment of phonons in QFT at large. We first analyze the Ward identity structure by means of standard QFT techniques, considering both spontaneous and explicit symmetry breaking. Next, by implementing holographic renormalization, we show that the same set of Ward identities holds in the holographic Q-lattice. Eventually, relying on the holographic and QFT results, we study the correlators realizing the symmetry breaking pattern and how they encode information about the low-energy spectrum.
Ultrafast modulation of electronic structure by coherent phonon excitations
Weisshaupt, J.; Rouzée, A.; Woerner, M.; Vrakking, M. J. J.; Elsaesser, T.; Shirley, E. L.; Borgschulte, A.
2017-02-01
Femtosecond x-ray absorption spectroscopy with a laser-driven high-harmonic source is used to map ultrafast changes of x-ray absorption by femtometer-scale coherent phonon displacements. In LiBH4, displacements along an Ag phonon mode at 10 THz are induced by impulsive Raman excitation and give rise to oscillatory changes of x-ray absorption at the Li K edge. Electron density maps from femtosecond x-ray diffraction data show that the electric field of the pump pulse induces a charge transfer from the BH4- to neighboring Li+ ions, resulting in a differential Coulomb force that drives lattice vibrations in this virtual transition state.
Jet formation in spallation of metal film from substrate under action of femtosecond laser pulse
Energy Technology Data Exchange (ETDEWEB)
Inogamov, N. A., E-mail: nailinogamov@googlemail.com [Russian Academy of Sciences, Landau Institute for Theoretical Physics (Russian Federation); Zhakhovskii, V. V. [Dukhov All-Russia Research Institute of Automatics (Russian Federation); Khokhlov, V. A. [Russian Academy of Sciences, Landau Institute for Theoretical Physics (Russian Federation)
2015-01-15
It is well known that during ablation by an ultrashort laser pulse, the main contribution to ablation of the substance is determined not by evaporation, but by the thermomechanical spallation of the substance. For identical metals and pulse parameters, the type of spallation is determined by film thickness d{sub f}. An important gauge is metal heating depth d{sub T} at the two-temperature stage, at which electron temperature is higher than ion temperature. We compare cases with d{sub f} < d{sub T} (thin film) and d{sub f} ≫ d{sub T} (bulk target). Radius R{sub L} of the spot of heating by an optical laser is the next (after d{sub f}) important geometrical parameter. The morphology of film bulging in cases where d{sub f} < d{sub T} on the substrate (blistering) changes upon a change in radius R{sub L} in the range from diffraction limit R{sub L} ∼ λ to high values of R{sub L} ≫ λ, where λ ∼ 1 μm is the wavelength of optical laser radiation. When d{sub f} < d{sub T}, R{sub L} ∼ λ, and F{sub abs} > F{sub m}, gold film deposited on the glass target acquires a cupola-shaped blister with a miniature frozen nanojet in the form of a tip on the circular top of the cupola (F{sub abs} and F{sub m} are the absorbed energy and the melting threshold of the film per unit surface area of the film). A new physical mechanism leading to the formation of the nanojet is proposed.
Phononic crystals of poroelastic spheres
Alevizaki, A.; Sainidou, R.; Rembert, P.; Morvan, B.; Stefanou, N.
2016-11-01
An extension of the layer-multiple-scattering method to phononic crystals of poroelastic spheres immersed in a fluid medium is developed. The applicability of the method is demonstrated on specific examples of close-packed fcc crystals of submerged water-saturated meso- and macroporous silica microspheres. It is shown that, by varying the pore size and/or the porosity, the transmission, reflection, and absorption spectra of finite slabs of these crystals are significantly altered. Strong absorption, driven by the slow waves in the poroelastic material and enhanced by multiple scattering, leads to negligible transmittance over an extended frequency range, which might be useful for practical applications in broadband acoustic shielding. The results are analyzed by reference to relevant phononic dispersion diagrams in the viscous and inertial coupling limits, and a consistent interpretation of the underlying physics is provided.
Edge phonons in black phosphorus
Ribeiro, H. B.; Villegas, C. E. P.; Bahamon, D. A.; Muraca, D.; Castro Neto, A. H.; de Souza, E. A. T.; Rocha, A. R.; Pimenta, M. A.; de Matos, C. J. S.
2016-07-01
Black phosphorus has recently emerged as a new layered crystal that, due to its peculiar and anisotropic crystalline and electronic band structures, may have important applications in electronics, optoelectronics and photonics. Despite the fact that the edges of layered crystals host a range of singular properties whose characterization and exploitation are of utmost importance for device development, the edges of black phosphorus remain poorly characterized. In this work, the atomic structure and behaviour of phonons near different black phosphorus edges are experimentally and theoretically studied using Raman spectroscopy and density functional theory calculations. Polarized Raman results show the appearance of new modes at the edges of the sample, and their spectra depend on the atomic structure of the edges (zigzag or armchair). Theoretical simulations confirm that the new modes are due to edge phonon states that are forbidden in the bulk, and originated from the lattice termination rearrangements.
Measuring phonons in protein crystals
Niessen, Katherine A.; Snell, Edward; Markelz, A. G.
2013-03-01
Using Terahertz near field microscopy we find orientation dependent narrow band absorption features for lysozyme crystals. Here we discuss identification of protein collective modes associated with the observed features. Using normal mode calculations we find good agreement with several of the measured features, suggesting that the modes arise from internal molecular motions and not crystal phonons. Such internal modes have been associated with protein function.
Cooling phonons with phonons: Acoustic reservoir engineering with silicon-vacancy centers in diamond
Kepesidis, K. V.; Lemonde, M.-A.; Norambuena, A.; Maze, J. R.; Rabl, P.
2016-12-01
We study a setup where a single negatively-charged silicon-vacancy center in diamond is magnetically coupled to a low-frequency mechanical bending mode and via strain to the high-frequency phonon continuum of a semiclamped diamond beam. We show that under appropriate microwave driving conditions, this setup can be used to induce a laser-cooling-like effect for the low-frequency mechanical vibrations, where the high-frequency longitudinal compression modes of the beam serve as an intrinsic low-temperature reservoir. We evaluate the experimental conditions under which cooling close to the quantum ground state can be achieved and describe an extended scheme for the preparation of a stationary entangled state between two mechanical modes. By relying on intrinsic properties of the mechanical beam only, this approach offers an interesting alternative for quantum manipulation schemes of mechanical systems, where otherwise efficient optomechanical interactions are not available.
Patimisco, Pietro; Scamarcio, Gaetano; Santacroce, Maria Vittoria; Spagnolo, Vincenzo; Vitiello, Miriam Serena; Dupont, Emmanuel; Laframboise, Sylvain R; Fathololoumi, Saeed; Razavipour, Ghasem S; Wasilewski, Zbigniew
2013-04-22
We measured the lattice and subband electronic temperatures of terahertz quantum cascade devices based on the optical phonon-scattering assisted active region scheme. While the electronic temperature of the injector state (j = 4) significantly increases by ΔT = T(e)(4) - T(L) ~40 K, in analogy with the reported values in resonant phonon scheme (ΔT ~70-110 K), both the laser levels (j = 2,3) remain much colder with respect to the latter (by a factor of 3-5) and share the same electronic temperature of the ground level (j = 1). The electronic population ratio n(2)/n(1) shows that the optical phonon scattering efficiently depopulates the lower laser level (j = 2) up to an electronic temperature T(e) ~180 K.
New Mid-IR Lasers Based on Rare-Earth-Doped Sulfide and Chloride Materials
Energy Technology Data Exchange (ETDEWEB)
Nostrand, M
2000-09-01
Applications in remote-sensing and military countermeasures have driven a need for compact, solid-state mid-IR lasers. Due to multi-phonon quenching, non-traditional hosts are needed to extend current solid-state, room-temperature lasing capabilities beyond {approx} 4 {micro}m. Traditional oxide and fluoride hosts have effective phonon energies in the neighborhood of 1000 cm{sup -1} and 500 cm{sup -1}, respectively. These phonons can effectively quench radiation above 2 and 4 {micro}m, respectively. Materials with lower effective phonon energies such as sulfides and chlorides are the logical candidates for mid-IR (4-10 {micro}m) operation. In this report, laser action is demonstrated in two such hosts, CaGa{sub 2}S{sub 4} and KPb{sub 2}Cl{sub 5}. The CaGa{sub 2}S{sub 4}:Dy{sup 3+} laser operating at 4.3 {micro}m represents the first sulfide laser operating beyond 2 {micro}m. The KPb{sub 2}Cl{sub 5}:Dy{sup 3+} laser operating at 2.4 {micro}m represents the first operation of a chloride-host laser in ambient conditions. Laser action is also reported for CaGa{sub 2}S{sub 4}:Dy{sup 3+} at 2.4 {micro}m, CaGa{sub 2}S{sub 4}:Dy{sup 3+} at 1.4 {micro}m, and KPb{sub 2}Cl{sub 5}:Nd{sup 3+} at 1.06 {micro}m. Both host materials have been fully characterized, including lifetimes, absorption and emission cross sections, radiative branching ratios, and radiative quantum efficiencies. Radiative branching ratios and radiative quantum efficiencies have been determined both by the Judd-Ofelt method (which is based on absorption measurements), and by a novel method described herein which is based on emission measurements. Modeling has been performed to predict laser performance, and a new method to determine emission cross section from slope efficiency and threshold data is developed. With the introduction and laser demonstration of rare-earth-doped CaGa{sub 2}S{sub 4} and KPb{sub 2}Cl{sub 5}, direct generation of mid-IR laser radiation in a solid-state host has been demonstrated. In
Blistering of film from substrate after action of ultrashort laser pulse
Inogamov, N. A.; Zhakhovsky, V. V.; Khokhlov, V. A.; Kuchmizhak, A. A.; Kudryashov, S. I.
2016-11-01
The goal of the paper is to explain experimental results concerning film blistering. Tightly focused diffraction limited ultrashort optical laser pulse illuminates a small spot at a surface of a thin metal film mounted upon a dielectric or semiconductor support (substrate). Film mechanically separates from substrate and form a cupola like bump in a rather narrow range of absorbed fluences. Below this range deformations inside the spot are negligible. While above the range the hole remains in a film in the irradiated spot. The paper presents physical model starting from absorption and two-temperature state and including, first, description of conductive redistribution of absorbed heat, melting, hydrodynamics of strong three-dimensional deformations of a moving film, and, second, freezing of molten metal.
Phonon-Assisted Resonant Tunnelling through a Triple-Quantum-Dot: a Phonon-Signal Detector
Institute of Scientific and Technical Information of China (English)
SHEN Xiao-Yun; DONG Bing; LEI Xiao-lin
2008-01-01
We study the effect of electron-phonon interaction on current and zero-frequency shot noise in resonant tunnelling through a series triple-quantum-dot coupling to a local phonon mode by means of a nonperturbative mapping technique along with the Green function formulation.By fixing the energy difference between the first two quantum dots to be equal to phonon frequency and sweeping the level of the third quantum dot,we find a largely enhanced current spectrum due to phonon effect,and in particular we predict current peaks corresponding to phonon-absorption and phonon-emission assisted resonant tunnelling processes,which show that this system can be acted as a sensitive phonon-signal detector or as a cascade phonon generator.
Resonant Enhancement of Coherent Phonons in Carbon Nanotubes Observed with Sub-10fs Time Resolution
Directory of Open Access Journals (Sweden)
Yanagi K.
2013-03-01
Full Text Available Using wavelength-resolved pump-probe spectroscopy with a sub-10-fs laser, we investigated resonant enhancement of radial breathing mode and G-mode coherent phonons in carbon nanotubes (CNTs, and successfully distinguished the electronic states of CNTs with different chiralities.
Electron-phonon interactions from first principles
Giustino, Feliciano
2017-01-01
This article reviews the theory of electron-phonon interactions in solids from the point of view of ab initio calculations. While the electron-phonon interaction has been studied for almost a century, predictive nonempirical calculations have become feasible only during the past two decades. Today it is possible to calculate from first principles many materials properties related to the electron-phonon interaction, including the critical temperature of conventional superconductors, the carrier mobility in semiconductors, the temperature dependence of optical spectra in direct and indirect-gap semiconductors, the relaxation rates of photoexcited carriers, the electron mass renormalization in angle-resolved photoelectron spectra, and the nonadiabatic corrections to phonon dispersion relations. In this article a review of the theoretical and computational framework underlying modern electron-phonon calculations from first principles as well as landmark investigations of the electron-phonon interaction in real materials is given. The first part of the article summarizes the elementary theory of electron-phonon interactions and their calculations based on density-functional theory. The second part discusses a general field-theoretic formulation of the electron-phonon problem and establishes the connection with practical first-principles calculations. The third part reviews a number of recent investigations of electron-phonon interactions in the areas of vibrational spectroscopy, photoelectron spectroscopy, optical spectroscopy, transport, and superconductivity.
Phonon counting and intensity interferometry of a nanomechanical resonator
Cohen, Justin D.; Meenehan, Seán M.; Maccabe, Gregory S.; Gröblacher, Simon; Safavi-Naeini, Amir H.; Marsili, Francesco; Shaw, Matthew D.; Painter, Oskar
2015-04-01
In optics, the ability to measure individual quanta of light (photons) enables a great many applications, ranging from dynamic imaging within living organisms to secure quantum communication. Pioneering photon counting experiments, such as the intensity interferometry performed by Hanbury Brown and Twiss to measure the angular width of visible stars, have played a critical role in our understanding of the full quantum nature of light. As with matter at the atomic scale, the laws of quantum mechanics also govern the properties of macroscopic mechanical objects, providing fundamental quantum limits to the sensitivity of mechanical sensors and transducers. Current research in cavity optomechanics seeks to use light to explore the quantum properties of mechanical systems ranging in size from kilogram-mass mirrors to nanoscale membranes, as well as to develop technologies for precision sensing and quantum information processing. Here we use an optical probe and single-photon detection to study the acoustic emission and absorption processes in a silicon nanomechanical resonator, and perform a measurement similar to that used by Hanbury Brown and Twiss to measure correlations in the emitted phonons as the resonator undergoes a parametric instability formally equivalent to that of a laser. Owing to the cavity-enhanced coupling of light with mechanical motion, this effective phonon counting technique has a noise equivalent phonon sensitivity of 0.89 +/- 0.05. With straightforward improvements to this method, a variety of quantum state engineering tasks using mesoscopic mechanical resonators would be enabled, including the generation and heralding of single-phonon Fock states and the quantum entanglement of remote mechanical elements.
Eichenfield, Matthew
The dynamic back-action caused by electromagnetic forces (radiation pressure) in optical and microwave cavities is of growing interest. Back-action cooling, for example, is being pursued as a means of achieving the quantum ground state of macroscopic mechanical oscillators. Work in the optical domain has revolved around millimeter- or micrometer-scale structures using the radiation pressure force. By comparison, in microwave devices, low-loss superconducting structures have been used for gradient-force-mediated coupling to a nanomechanical oscillator of picogram mass. In this thesis, two different nanometer-scale structures that use combinations of gradient and radiation pressure optical forces are described theoretically and demonstrated experimentally. These structures merge the fields of cavity optomechanics and nanomechanics into nano-optomechanical systsms (NOMS). The first device, the “Zipper” optomechanical cavity, consists of a pair of doubly-clamped nanoscale beams separated by approximately 100 nanometers, each beam having a mass of 20 picograms and being patterned with a quasi-1D photonic crystal bandgap cavity. The optical mode of the coupled system is exquisitely sensitive to differential motion of the beams, producing optomechanical coupling right at the fundamental limit set by optical diffraction. The mechanical modes of the beam probed with a background sensitivity only a factor of 4 above the standard quantum limit, and the application of less than a milliwatt of optical power is shown to increase the mechanical rigidity of the system by almost an order of magnitude. The second device focuses on just one of the doubly-clamped nanoscale beams of the Zipper. We show that, in addition to a photonic bandgap cavity, the periodic patterning of the beam also produces a phononic bandgap cavity with localized mechanical modes having frequencies in the microwave regime. We call these photonic and phononic crystal bandgap cavities optomechanical crystals
Dynamical stabilization by phonon-phonon interaction exemplified in cubic zirconia
Energy Technology Data Exchange (ETDEWEB)
Souvatsos, [etrps G [Los Alamos National Laboratory; Rudin, Sven P [Los Alamos National Laboratory
2008-01-01
Cubic zirconia exhibits a soft phonon mode (X{sup -}{sub 2}), which becomes dynamically unstable at low temperatures. Previous ab initio invest.igations into the temperature-induced stabilization of the soft mode treated it as an independent anharmonic oscillator. Calculations presented here, using the self consistent ab initio lattice dynamical (SCAILD) method to evaluate the phonons at 2570 K, show that the soft mode should not be treated independently of other phonon modes. Phonon-phonon interactions stabilize the X{sup -}{sub 2} mode. Furthermore, the effective potential experienced by the mode takes on a quadratic form.
Splash, pop, sizzle: Information processing with phononic computing
Directory of Open Access Journals (Sweden)
Sophia R. Sklan
2015-05-01
Full Text Available Phonons, the quanta of mechanical vibration, are important to the transport of heat and sound in solid materials. Recent advances in the fundamental control of phonons (phononics have brought into prominence the potential role of phonons in information processing. In this review, the many directions of realizing phononic computing and information processing are examined. Given the relative similarity of vibrational transport at different length scales, the related fields of acoustic, phononic, and thermal information processing are all included, as are quantum and classical computer implementations. Connections are made between the fundamental questions in phonon transport and phononic control and the device level approach to diodes, transistors, memory, and logic.
Interaction of coherent phonons with defects and elementary excitations
Energy Technology Data Exchange (ETDEWEB)
Hase, Muneaki [Institute of Applied Physics, University of Tsukuba, 1-1-1 Tennodai, Tsukuba 305-8573 (Japan); Kitajima, Masahiro, E-mail: mhase@bk.tsukuba.ac.j, E-mail: kitaji@nda.ac.j [Department of Applied Physics, School of Applied Science, National Defense Academy of Japan, Hashirimizu 1-10-20, Yokosuka, Kanagawa 239-8686 (Japan)
2010-02-24
We present an overview of the feasibility of using coherent phonon spectroscopy to study interaction dynamics of excited lattice vibrations with their environments. By exploiting the features of coherent phonons with a pump-probe technique, one can study lattice motions in a sub-picosecond time range. The dephasing properties tell us not only about interaction dynamics with carriers (electrons and holes) or thermal phonons but also about point defects in crystals. Modulations of the coherent phonon amplitude by more than two modes are closely related to phonon-carrier or phonon-phonon interferences. Related to this phenomenon, formation of coherent phonons at higher harmonics gives direct evidence for phonon-phonon couplings. A combined study of coherent phonons and ultrafast carrier response can be useful for understanding phonon-carrier interaction dynamics. For metals like zinc, nonequilibrium electrons may dominate the dynamics of both relaxation and generation of coherent phonons. The frequency chirp of coherent phonons can be a direct measure of how and when phonon-phonon and phonon-carrier couplings occur. Carbon nanotubes show some complicated behavior due to the existence of many modes with different symmetries, resulting in superposition or interference. To illustrate one of the most interesting applications, the selective excitation of specific phonon modes through the use of a pulse train technique is shown. (topical review)
Phonon dispersion relation of liquid metals
Indian Academy of Sciences (India)
P B Thakor; P N Gajjar; A R Jani
2009-06-01
The phonon dispersion curves of some liquid metals, viz. Na ( = 1), Mg ( = 2), Al ( = 3) and Pb ( = 4), have been computed using our model potential. The charged hard sphere (CHS) reference system is applied to describe the structural information. Our model potential along with CHS reference system is capable of explaining the phonon dispersion relation for monovalent, divalent, trivalent and tetravalent liquid metals.
Anharmonic phonons and high-temperature superconductivity
Energy Technology Data Exchange (ETDEWEB)
Crespi, V.H.; Cohen, M.L. (Department of Physics, University of California at Berkeley, and Materials Sciences Division, Lawrence Berkeley Laboratory, Berkeley, California 94720 (United States))
1993-07-01
We examine a simple model of anharmonic phonons with application to the superconducting isotope effect. Linear and quadratic electron-phonon coupling are considered for various model potentials. The results of the model calculations are compared with the high-temperature superconductors La[sub 2[minus][ital x
Energy Technology Data Exchange (ETDEWEB)
Dudetskiy, V Yu; Lariontsev, E G; Chekina, S N [Department of Physics, M.V. Lomonosov Moscow State University (Russian Federation)
2014-09-30
The effect of pump noise on the synchronisation of selfmodulation oscillations in a solid-state ring laser with periodic pump modulation is studied numerically and experimentally. It is found that, in contrast to desynchronisation that usually occurs under action of noise in the case of 1/1 synchronisation of self-oscillations by a periodic signal, the effect of noise on 1/2 synchronisation may be positive, namely, at a sufficiently low intensity, pump noise is favourable for synchronisation of self-oscillations, for narrowing of their spectrum, and for increasing the signal-to-noise ratio. (lasers)
Isotope effect on electron-phonon interaction in the multiband superconductor MgB2
Mou, Daixiang; Manni, Soham; Taufour, Valentin; Wu, Yun; Huang, Lunan; Bud'ko, S. L.; Canfield, P. C.; Kaminski, Adam
2016-04-01
We investigate the effect of isotope substitution on the electron-phonon interaction in the multiband superconductor MgB2 using tunable laser-based angle-resolved photoemission spectroscopy. The kink structure around 70 meV in the σ band, which is caused by electron coupling to the E2 g phonon mode, is shifted to higher binding energy by ˜3.5 meV in Mg 10B2 and the shift is not affected by superconducting transition. These results serve as the benchmark for investigations of isotope effects in known, unconventional superconductors and newly discovered superconductors where the origin of pairing is unknown.
von Reppert, A; Pudell, J; Koc, A; Reinhardt, M; Leitenberger, W; Dumesnil, K; Zamponi, F; Bargheer, M
2016-09-01
We present a temperature and fluence dependent Ultrafast X-Ray Diffraction study of a laser-heated antiferromagnetic dysprosium thin film. The loss of antiferromagnetic order is evidenced by a pronounced lattice contraction. We devise a method to determine the energy flow between the phonon and spin system from calibrated Bragg peak positions in thermal equilibrium. Reestablishing the magnetic order is much slower than the cooling of the lattice, especially around the Néel temperature. Despite the pronounced magnetostriction, the transfer of energy from the spin system to the phonons in Dy is slow after the spin-order is lost.
Directory of Open Access Journals (Sweden)
A. von Reppert
2016-09-01
Full Text Available We present a temperature and fluence dependent Ultrafast X-Ray Diffraction study of a laser-heated antiferromagnetic dysprosium thin film. The loss of antiferromagnetic order is evidenced by a pronounced lattice contraction. We devise a method to determine the energy flow between the phonon and spin system from calibrated Bragg peak positions in thermal equilibrium. Reestablishing the magnetic order is much slower than the cooling of the lattice, especially around the Néel temperature. Despite the pronounced magnetostriction, the transfer of energy from the spin system to the phonons in Dy is slow after the spin-order is lost.
Phononic crystals and elastodynamics: Some relevant points
Energy Technology Data Exchange (ETDEWEB)
Aravantinos-Zafiris, N. [Dept. of Materials Science, University of Patras, Patras 26504 (Greece); Department of Sound and Musical Instruments Technology, Ionian Islands Technological Educational Institute, Lixouri, 28200 (Greece); Sigalas, M. M. [Dept. of Materials Science, University of Patras, Patras 26504 (Greece); Kafesaki, M. [Institute of Electronic Structure and Laser (IESL), Foundation for Research and Technology, Hellas (FORTH), P.O. Box 1387, 70013 Heraklion, Crete (Greece); Dept. of Materials Science and Technology, Univ. of Crete (Greece); Economou, E. N. [Institute of Electronic Structure and Laser (IESL), Foundation for Research and Technology, Hellas (FORTH), P.O. Box 1387, 70013 Heraklion, Crete (Greece); Dept. of Physics, Univ. of Crete (Greece)
2014-12-15
In the present paper we review briefly some of the first works on wave propagation in phononic crystals emphasizing the conditions for the creation of acoustic band-gaps and the role of resonances to the band-gap creation. We show that useful conclusions in the analysis of phononic band gap structures can be drawn by considering the mathematical similarities of the basic classical wave equation (Helmholtz equation) with Schrödinger equation and by employing basic solid state physics concepts and conclusions regarding electronic waves. In the second part of the paper we demonstrate the potential of phononic systems to be used as elastic metamaterials. This is done by demonstrating negative refraction in phononic crystals and subwavelength waveguiding in a linear chain of elastic inclusions, and by proposing a novel structure with close to pentamode behavior. Finally the potential of phononic structures to be used in liquid sensor applications is discussed and demonstrated.
Ultrafast Structure Switching through Nonlinear Phononics
Juraschek, D. M.; Fechner, M.; Spaldin, N. A.
2017-02-01
We describe a mechanism by which nonlinear phononics allows ultrafast coherent and directional control of transient structural distortions. With ErFeO3 as a model system, we use density functional theory to calculate the structural properties as input into an anharmonic phonon model that describes the response of the system to a pulsed optical excitation. We find that the trilinear coupling of two orthogonal infrared-active phonons to a Raman-active phonon causes a transient distortion of the lattice. In contrast to the quadratic-linear coupling that has been previously explored, the direction of the distortion is determined by the polarization of the exciting light, introducing a novel mechanism for nonlinear phononic switching. Since the occurrence of the coupling is determined by the symmetry of the system we propose that it is a universal feature of orthorhombic and tetragonal perovskites.
Phononic crystals and elastodynamics: Some relevant points
Directory of Open Access Journals (Sweden)
N. Aravantinos-Zafiris
2014-12-01
Full Text Available In the present paper we review briefly some of the first works on wave propagation in phononic crystals emphasizing the conditions for the creation of acoustic band-gaps and the role of resonances to the band-gap creation. We show that useful conclusions in the analysis of phononic band gap structures can be drawn by considering the mathematical similarities of the basic classical wave equation (Helmholtz equation with Schrödinger equation and by employing basic solid state physics concepts and conclusions regarding electronic waves. In the second part of the paper we demonstrate the potential of phononic systems to be used as elastic metamaterials. This is done by demonstrating negative refraction in phononic crystals and subwavelength waveguiding in a linear chain of elastic inclusions, and by proposing a novel structure with close to pentamode behavior. Finally the potential of phononic structures to be used in liquid sensor applications is discussed and demonstrated.
The phonon Hall effect: theory and application
Energy Technology Data Exchange (ETDEWEB)
Zhang Lifa; Wang Jiansheng; Li Baowen [Department of Physics and Centre for Computational Science and Engineering, National University of Singapore, Singapore 117542 (Singapore); Ren Jie [NUS Graduate School for Integrative Sciences and Engineering, Singapore 117456 (Singapore)
2011-08-03
We present a systematic theory of the phonon Hall effect in a ballistic crystal lattice system, and apply it on the kagome lattice which is ubiquitous in various real materials. By proposing a proper second quantization for the non-Hermitian in the polarization-vector space, we obtain a new heat current density operator with two separate contributions: the normal velocity responsible for the longitudinal phonon transport, and the anomalous velocity manifesting itself as the Hall effect of transverse phonon transport. As exemplified in kagome lattices, our theory predicts that the direction of Hall conductivity at low magnetic field can be reversed by tuning the temperatures, which we hope can be verified by experiments in the future. Three phonon-Hall-conductivity singularities induced by phonon-band-topology change are discovered as well, which correspond to the degeneracies at three different symmetric center points, {Gamma}, K, X, in the wavevector space of the kagome lattice.
Ab initio phonon coupling and optical response of hot electrons in plasmonic metals
Brown, Ana M; Narang, Prineha; Goddard, William A; Atwater, Harry A
2016-01-01
Ultrafast laser measurements probe the non-equilibrium dynamics of excited electrons in metals with increasing temporal resolution. Electronic structure calculations can provide a detailed microscopic understanding of hot electron dynamics, but a parameter-free description of pump-probe measurements has not yet been possible, despite intensive research, because of the phenomenological treatment of electron-phonon interactions. We present ab initio predictions of the electron-temperature dependent heat capacities and electron-phonon coupling coefficients of plasmonic metals. We find substantial differences from free-electron and semi-empirical estimates, especially in noble metals above transient electron temperatures of 2000 K, because of the previously-neglected strong dependence of electron-phonon matrix elements on electron energy. We also present first-principles calculations of the electron-temperature dependent dielectric response of hot electrons in plasmonic metals, including direct interband and phon...
Longitudinal polar optical phonons in InN/GaN single and double het- erostructures
Energy Technology Data Exchange (ETDEWEB)
Ardali, Sukru; Tiras, Engin [Department of Physics, Faculty of Science, Anadolu University, Yunus Emre Campus, Eskisehir 26470 (Turkey); Gunes, Mustafa; Balkan, Naci [School of Computer Science and Electronic Engineering, University of Essex, Wivenhoe Park, Colchester CO4 3SQ (United Kingdom); Ajagunna, Adebowale Olufunso; Iliopoulos, Eleftherios; Georgakilas, Alexandros [Microelectronics Research Group, IESL, FORTH and Physics Department, University of Crete, P.O. Box 1385, 71110 Heraklion-Crete (Greece)
2011-05-15
Longitudinal optical phonon energy in InN epi-layers has been determined independently from the Raman spectroscopy and temperature dependent Hall mobility measurements. Raman spectroscopy technique can be used to obtain directly the LO energy where LO phonon scattering dominates transport at high temperature. Moreover, the Hall mobility is determined by the scattering of electrons with LO phonons so the data for the temperature dependence of Hall mobility have been used to calculate the effective energy of longitudinal optical phonons.The samples investigated were (i) single heterojunction InN with thicknesses of 1.08, 2.07 and 4.7 {mu}m grown onto a 40 nm GaN buffer and (ii) GaN/InN/AlN double heterojunction samples with InN thicknesses of 0.4, 0.6 and 0.8 {mu}m. Hall Effect measurements were carried out as a function of temperature in the range between T = 1.7 and 275 K at fixed magnetic and electric fields. The Raman spectra were obtained at room temperature. In the experiments, the 532 nm line of a nitrogen laser was used as the excitation source and the light was incident onto the samples along of the growth direction (c-axis). The results, obtained from the two independent techniques suggest the following: (1) LO phonon energies obtained from momentum relaxation experiments are generally slightly higher than those obtained from the Raman spectra. (2) LO phonon energy for the single heterojunctions does not depend on the InN thickness. (3) In double heterostructures, with smaller InN thicknesses and hence with increased strain, LO phonon energy increases by 3% (experimental accuracy is < 1%) when the InN layer thickness increases from 400 to 800 nm (copyright 2011 WILEY-VCH Verlag GmbH and Co. KGaA, Weinheim) (orig.)
Single-photon indistinguishability: influence of phonons
DEFF Research Database (Denmark)
Nielsen, Per Kær; Lodahl, Peter; Jauho, Antti-Pekka;
2012-01-01
Recent years have demonstrated that the interaction with phonons plays an important role in semiconductor based cavity QED systems [2], consisting of a quantum dot (QD) coupled to a single cavity mode [Fig. 1(a)], where the phonon interaction is the main decoherence mechanism. Avoiding decoherence...... of photons emitted from a solid-state cavity QED system. Our model rigorously describes non-Markovian effects to all orders in the phonon coupling constant, being based on an exact diagonalization procedure accounting for the time evoluiton of one-time and two-time photon correlation funcitons. We compare...
Acoustic superfocusing by solid phononic crystals
Zhou, Xiaoming; Assouar, M. Badreddine; Oudich, Mourad
2014-12-01
We propose a solid phononic crystal lens capable of acoustic superfocusing beyond the diffraction limit. The unit cell of the crystal is formed by four rigid cylinders in a hosting material with a cavity arranged in the center. Theoretical studies reveal that the solid lens produces both negative refraction to focus propagating waves and surface states to amplify evanescent waves. Numerical analyses of the superfocusing effect of the considered solid phononic lens are presented with a separated source excitation to the lens. In this case, acoustic superfocusing beyond the diffraction limit is evidenced. Compared to the fluid phononic lenses, the solid lens is more suitable for ultrasonic imaging applications.
One-dimensional hypersonic phononic crystals.
Gomopoulos, N; Maschke, D; Koh, C Y; Thomas, E L; Tremel, W; Butt, H-J; Fytas, G
2010-03-10
We report experimental observation of a normal incidence phononic band gap in one-dimensional periodic (SiO(2)/poly(methyl methacrylate)) multilayer film at gigahertz frequencies using Brillouin spectroscopy. The band gap to midgap ratio of 0.30 occurs for elastic wave propagation along the periodicity direction, whereas for inplane propagation the system displays an effective medium behavior. The phononic properties are well captured by numerical simulations. The porosity in the silica layers presents a structural scaffold for the introduction of secondary active media for potential coupling between phonons and other excitations, such as photons and electrons.
Gastaud, C.; Redon, M.; Belland, P.; Fourrier, M.
1984-06-01
This paper reports the first use of a N2O laser for optically pumping vinyl halides, to obtain new cw submillimeter laser lines. Eighteen far-infrared (FIR) emissions have been observed in vinyl chloride, twenty five in vinyl bromide and thirty eight in vinyl flouride.
Kuleev, I G
2001-01-01
The effect of normal processes of the phonon-phonon scattering on the thermal conductivity of the germanium crystals with various isotopic disorder degrees is considered. The phonon pulse redistribution in the normal scattering processes both inside each oscillatory branch (the Simons mechanism) and between various phonon oscillatory branches (the Herring mechanism) is accounted for. The contributions of the longitudinal and cross-sectional phonons drift motion into the thermal conductivity are analyzed. It is shown that the pulse redistribution in the Herring relaxation mechanism leads to essential suppression of the longitudinal phonons drift motion in the isotopically pure germanium crystals. The calculations results of thermal conductivity for the Herring relaxation mechanism agree well with experimental data on the germanium crystals with various isotopic disorder degrees
Investigation of the Phonon Frequency Shifts in ZnO Quantum Dots
Alim, Khan A.
2005-03-01
Nanostructures made of ZnO have recently attracted attention due to their proposed applications in low-voltage and short-wavelength electro-optical devices. However, the origin of the observed phonon frequency shifts in such nanostructures is not always understood. We carried out both resonant and non-resonant Raman measurements for 20 nm-diameter ZnO quantum dots (QDs) and bulk ZnO reference samples [1]. A comparison with a recently developed theory [2], allowed us to clarify the origin of the phonon frequency shifts in ZnO QDs. It was found that the phonon confinement results in phonon frequency shifts of only few cm-1. At the same time, the UV laser heating of the QD ensemble was found to induce a large red shift of phonon frequencies for up to 14 cm-1. The authors acknowledge the support of MARCO and its Functional Engineered Nano Architectonics (FENA) Focus Center. [1] K.A. Alim, V.A. Fonoberov, and A.A. Balandin, Appl. Phys. Lett., in review (2004). [2] V.A. Fonoberov and A.A. Balandin, Phys. Stat. Solidi C 1, 2650 (2004); cond-mat/0405681; cond-mat/0411742.
Effects of phonon-phonon coupling on properties of pygmy resonance in 124-132Sn
Directory of Open Access Journals (Sweden)
Voronov V. V.
2012-12-01
Full Text Available Starting from an effective Skyrme interaction we study effects of phonon-phonon coupling on the low-energy electric dipole response in 124-132Sn. The QRPA calculations are performed within a finite rank separable approximation. The inclusion of two-phonon configurations gives a considerable contribution to low-lying strength. Comparison with available experimental data shows a reasonable agreement for the low-energy E1 strength distribution.
Passeron, T
2012-12-01
Lasers are a very effective approach for treating many hyperpigmented lesions. They are the gold standard treatment for actinic lentigos and dermal hypermelanocytosis, such as Ota nevus. Becker nevus, hyperpigmented mosaicisms, and lentigines can also be successfully treated with lasers, but they could be less effective and relapses can be observed. However, lasers cannot be proposed for all types of hyperpigmentation. Thus, freckles and café-au-lait macules should not be treated as the relapses are nearly constant. Due to its complex pathophysiology, melasma has a special place in hyperpigmented dermatoses. Q-switched lasers (using standard parameters or low fluency) should not be used because of consistent relapses and the high risk of post-inflammatory hyperpigmentation. Paradoxically, targeting the vascular component of the melasma lesion with lasers could have a beneficial effect. However, these results have yet to be confirmed. In all cases, a precise diagnosis of the type of hyperpigmentation is mandatory before any laser treatment, and the limits and the potential side effects of the treatment must be clearly explained to patients.
Passeron, T
2012-11-01
Lasers are a very effective approach for treating many hyperpigmented lesions. They are the gold standard treatment for actinic lentigos and dermal hypermelanocytosis, such as Ota nevus. Becker nevus, hyperpigmented mosaicisms, and lentigines can also be successfully treated with lasers, but they could be less effective and relapses can be observed. However, lasers cannot be proposed for all types of hyperpigmentation. Thus, freckles and café-au-lait macules should not be treated as the relapses are nearly constant. Due to its complex pathophysiology, melasma has a special place in hyperpigmented dermatoses. Q-switched lasers (using standard parameters or low fluency) should not be used because of consistent relapses and the high risk of post-inflammatory hyperpigmentation. Paradoxically, targeting the vascular component of the melasma lesion with lasers could have a beneficial effect. However, these results have yet to be confirmed. In all cases, a precise diagnosis of the type of hyperpigmentation is mandatory before any laser treatment, and the limits and the potential side effects of the treatment must be clearly explained to patients.
Yudistira, D; Boes, A; Djafari-Rouhani, B; Pennec, Y; Yeo, L Y; Mitchell, A; Friend, J R
2014-11-21
We theoretically and experimentally demonstrate the existence of complete surface acoustic wave band gaps in surface phonon-polariton phononic crystals, in a completely monolithic structure formed from a two-dimensional honeycomb array of hexagonal shape domain-inverted inclusions in single crystal piezoelectric Z-cut lithium niobate. The band gaps appear at a frequency of about twice the Bragg band gap at the center of the Brillouin zone, formed through phonon-polariton coupling. The structure is mechanically, electromagnetically, and topographically homogeneous, without any physical alteration of the surface, offering an ideal platform for many acoustic wave applications for photonics, phononics, and microfluidics.
Theory of temperature dependent phonon-renormalized properties
Monserrat, Bartomeu; Conduit, G. J.; Needs, R. J.
2013-01-01
We present a general harmonic theory for the temperature dependence of phonon-renormalized properties of solids. Firstly, we formulate a perturbation theory in phonon-phonon interactions to calculate the phonon renormalization of physical quantities. Secondly, we propose two new schemes for extrapolating phonon zero-point corrections from temperature dependent data that improve the accuracy by an order of magnitude compared to previous approaches. Finally, we consider the low-temperature limi...
Acoustic and optical phonons in metallic diamond
Directory of Open Access Journals (Sweden)
M. Hoesch, T. Fukuda, T. Takenouchi, J.P. Sutter, S. Tsutsui, A.Q.R. Baron, M. Nagao, Y. Takano, H. Kawarada and J. Mizuki
2006-01-01
Full Text Available The dispersion of acoustic and optical phonons in highly boron-doped diamond has been measured by inelastic X-ray scattering at an energy resolution of 6.4 meV. The sample is doped in the metallic regime and shows superconductivity below 4.2 K (midpoint. The data are compared to pure and nitrogen-doped diamond that represent the non-metallic state. No difference is found for the acoustic phonons in the three samples, while the optical phonons show a shift of the dispersion (softening in qualitative agreement with earlier results from Raman spectroscopy. The presence of boron and nitrogen incorporated into the diamond lattice leads to structural disorder. Evidence for this is found both in the observation of otherwise symmetry-forbidded Bragg intensity at (0 0 2 and intensity from acoustic phonon modes in the vicinity of (0 0 2.
Influence of phonons on semiconductor quantum emission
Energy Technology Data Exchange (ETDEWEB)
Feldtmann, Thomas
2009-07-06
A microscopic theory of interacting charge carriers, lattice vibrations, and light modes in semiconductor systems is presented. The theory is applied to study quantum dots and phonon-assisted luminescence in bulk semiconductors and heterostructures. (orig.)
Acoustic Phonon Thermal Transport through a Nanostructure
Institute of Scientific and Technical Information of China (English)
LI Wen-Xia; LIU Tian-Yu; LIU Chang-Long
2006-01-01
@@ Using the scattering matrix method, we investigate the thermal transport in a nanostructure at low temperatures.It is found that phonon transport exhibits some novel and interesting features: resonant transmission, resonant reflection, and small thermal conductance.
Ab initio phonon coupling and optical response of hot electrons in plasmonic metals
Brown, Ana M.; Sundararaman, Ravishankar; Narang, Prineha; Goddard, William A.; Atwater, Harry A.
2016-08-01
Ultrafast laser measurements probe the nonequilibrium dynamics of excited electrons in metals with increasing temporal resolution. Electronic structure calculations can provide a detailed microscopic understanding of hot electron dynamics, but a parameter-free description of pump-probe measurements has not yet been possible, despite intensive research, because of the phenomenological treatment of electron-phonon interactions. We present ab initio predictions of the electron-temperature dependent heat capacities and electron-phonon coupling coefficients of plasmonic metals. We find substantial differences from free-electron and semiempirical estimates, especially in noble metals above transient electron temperatures of 2000 K, because of the previously neglected strong dependence of electron-phonon matrix elements on electron energy. We also present first-principles calculations of the electron-temperature dependent dielectric response of hot electrons in plasmonic metals, including direct interband and phonon-assisted intraband transitions, facilitating complete theoretical predictions of the time-resolved optical probe signatures in ultrafast laser experiments.
Phonon Cooling by an Optomechanical Heat Pump.
Dong, Ying; Bariani, F; Meystre, P
2015-11-27
We propose and analyze theoretically a cavity optomechanical analog of a heat pump that uses a polariton fluid to cool mechanical modes coupled to a single precooled phonon mode via external modulation of the substrate of the mechanical resonator. This approach permits us to cool phonon modes of arbitrary frequencies not limited by the cavity-optical field detuning deep into the quantum regime from room temperature.
Stem, Michelle R.
2016-05-01
The purpose of the present research was to investigate an intense violet shift displayed by a non-toxic, natural silicate material with a highly ordered nanostructure. The material displayed an unexpected, nonlinear 2:3 photon-phonon anti-Stokes upconversion while photonically, electronically, and thermally isolated. Conducted aphotonically and at ambient temperatures, the specimen upconverted a low-power, 650 nm constant wave red laser to an internally highly dispersed 433 nm violet wavelength. The strong dispersion was largely due to nearly total internal reflection of the laser. The upconversion had an efficiency of about 78 %, based on specimen volume, with no detectable thermal variance. The 2:3 anti-Stokes upconversion displayed by this material is likely the result of a previously unknown photon-phonon evanescence response that amplified the energy of a portion of the incident laser photons. Thus, a portion of the incident laser photons were upconverted, and the material converted another portion into an amplified energy that caused the upconversion. Internal micro-lasing appeared to be a means of photon-phonon evanescent energy redistribution, enabling dispersed photonic upconversion. Additional analyses also found an unexpectedly rhythmic photonic structure in spectrophotometric scans, polariscopic color changing, and previously undocumented ultraviolet responses.
Energy Technology Data Exchange (ETDEWEB)
Vinokhodov, A Yu; Krivokorytov, M S [EUV Labs, Ltd., Troitsk, Moscow (Russian Federation); Koshelev, K N; Krivtsun, V M; Sidelnikov, Yu V; Medvedev, V V; Kompanets, V O; Melnikov, A A; Chekalin, S V [Institute of Spectroscopy, Russian Academy of Sciences, Troitsk, Moscow (Russian Federation)
2016-01-31
We report the results of studying the dynamics of deformation and fragmentation of liquid-metal droplets under the action of ultrashort laser pulses. The experiments have been performed to optimise the shape of the droplet target used in extreme ultraviolet (EUV) radiation sources based on the laser-produced plasma using the pre-pulse technology. The pre-pulse is generated by a system incorporating a master Ti : sapphire oscillator and a regenerative amplifier, allowing one to vary the pulse duration from 50 fs to 50 ps. The power density of laser radiation at the droplet target, averaged over the pulse duration and spatial coordinates, has reached 3 × 10{sup 15} W cm{sup -2}. The production of liquid-metal droplets has been implemented by means of a droplet generator based on a nozzle with a ring piezoceramic actuator. The droplet material is the eutectic indium – tin alloy. The droplet generator could operate in the droplet and jet regime with a maximal rate of stable operation 5 and 150 kHz, respectively. The spatial stability of droplet position σ = 1% – 2% of its diameter is achieved. The size of the droplets varied within 30 – 70 μm, their velocity was 2 – 8 m s{sup -1} depending on the operation regime. (interaction of laser radiation with matter. laser plasma)
Squeezed Phonons: Modulating Quantum Fluctuations of Atomic Displacements.
Hu, Xuedong; Nori, Franco
1997-03-01
We have studied phonon squeezed states and also put forward several proposals for their generation(On phonon parametric process, X. Hu and F. Nori, Phys. Rev. Lett. 76), 2294 (1996); on polariton mechanism, X. Hu and F. Nori, Phys. Rev. B 53, 2419 (1996); on second-order Raman scattering, X. Hu and F. Nori, preprint.. Here, we compare the relative merits and limitations of these approaches, including several factors that will limit the amount of phonon squeezing. In particular, we investigate the effect of the initial thermal states on the phonon modes. Using a model for the phonon density matrix, we also study the mixing of the phonon squeezed states with thermal states, which describes the decay of the phonon coherence. Finally, we calculate the maximum possible squeezing from a phonon parametric process limited by phonon decay.
Rury, Aaron S.
2016-06-01
This study reports experimental, computational, and theoretical evidence for a previously unobserved coherent phonon-phonon interaction in an organic solid that can be described by the application of Fano's analysis to a case without the presence of a continuum. Using Raman spectroscopy of the hydrogen-bonded charge-transfer material quinhydrone, two peaks appear near 700 cm-1 we assign as phonons whose position and line-shape asymmetry depend on the sample temperature and light scattering excitation energy. Density functional theory calculations find two nearly degenerate phonons possessing frequencies near the values found in experiment that share similar atomic motion out of the aromatic plane of electron donor and acceptor molecules of quinhydrone. Further analytical modeling of the steady-state light scattering process using the Peierls-Hubbard Hamiltonian and time-dependent perturbation theory motivates assignment of the physical origin of the asymmetric features of each peak's line shape to an interaction between two discrete phonons via nonlinear electron-phonon coupling. In the context of analytical model results, characteristics of the experimental spectra upon 2.33 eV excitation of the Raman scattering process are used to qualify the temperature dependence of the magnitude of this coupling in the valence band of quinhydrone. These results broaden the range of phonon-phonon interactions in materials in general while also highlighting the rich physics and fundamental attributes specific to organic solids that may determine their applicability in next generation electronics and photonics technologies.
Energy Technology Data Exchange (ETDEWEB)
Karas, V. I., E-mail: karas@kipt.kharkov.ua; Vlasenko, A. M.; Sokolenko, V. I. [National Academy of Sciences of Ukraine, National Science Center “Kharkov Institute of Physics and Technology,” (Ukraine); Zakharov, V. E. [Russian Academy of Sciences, Lebedev Physical Institute (Russian Federation)
2015-09-15
We present the results of a kinetic analysis of nonequilibrium dynamics of the electron–phonon system of a crystal in a strong electric field based on the proposed method of numerically solving a set of Boltzmann equations for electron and phonon distribution functions without expanding the electron distribution function into a series in the phonon energy. It is shown that the electric field action excites the electron subsystem, which by transferring energy to the phonon subsystem creates a large amount of short-wave phonons that effectively influence the lattice defects (point, lines, boundaries of different phases), which results in a redistribution of and decrease in the lattice defect density, in damage healing, in a decrease in the local peak stress, and a decrease in the degradation level of the construction material properties.
Davidov, Nicolay N.; Kudaev, Serge V.
1999-01-01
Researchers of damage formation in processes in glass are directed on studying the interaction mechanisms of powerful impulses of penetrating laser radiation with materials for the purpose of improvement of optical components resistance. However, the processes of glass structure defects formation as local areas with low factor of visible light admittance can find application in a final glassware processing. Application of treatment modes, using these effects, allows: to increase art expression of decorative glassware for furnish of buildings interior; to solve some problems of manufacturing counter devices, and also indication devices of electronic instruments. Mathematical models of defect formation processes in optically transparent materials under an action of powerful pulses of laser radiation are necessary for development of control principles of glass treatment.
Phonon surface mapping of graphite: Disentangling quasi-degenerate phonon dispersions
Grüneis, A.; Serrano, J.; Bosak, A.; Lazzeri, M.; Molodtsov, S. L.; Wirtz, L.; Attaccalite, C.; Krisch, M.; Rubio, A.; Mauri, F.; Pichler, T.
2009-08-01
The two-dimensional mapping of the phonon dispersions around the K point of graphite by inelastic x-ray scattering is provided. The present work resolves the longstanding issue related to the correct assignment of transverse and longitudinal phonon branches at K . We observe an almost degeneracy of the three TO-, LA-, and LO-derived phonon branches and a strong phonon trigonal warping. Correlation effects renormalize the Kohn anomaly of the TO mode, which exhibits a trigonal warping effect opposite to that of the electronic band structure. We determined the electron-phonon coupling constant to be 166(eV/Å)2 in excellent agreement to GW calculations. These results are fundamental for understanding angle-resolved photoemission, double-resonance Raman and transport measurements of graphene-based systems.
Heating of nonequilibrium electrons by laser radiation in solid transparent dielectrics
Nikiforov, A. M.; Epifanov, A. S.; Garnov, S. V.
2011-01-01
A computer simulation of the heating of nonequilibrium electrons by an intense high-frequency electromagnetic field leading to the bulk damage of solid transparent dielectrics under single irradiation has been carried out. The dependences of the avalanche ionization rate on threshold field strength have been derived. Using the Fokker-Planck equation with a flux-doubling boundary condition is shown to lead to noticeable errors even at a ratio of the photon energy to the band gap ˜0.1. The series of dependences of the critical fields on pulse duration have been constructed for various initial lattice temperatures and laser wavelengths, which allow the electron avalanche to be identified as a limiting breakdown mechanism. The ratio of the energy stored in the electron subsystem to the excess (with respect to the equilibrium state) energy of the phonon subsystem by the end of laser pulse action has been calculated both with and without allowance for phonon heating. The influence of phonon heating on the impact avalanche ionization rate is analyzed.
Ionizing particle detection based on phononic crystals
Aly, Arafa H.; Mehaney, Ahmed; Eissa, Mostafa F.
2015-08-01
Most conventional radiation detectors are based on electronic or photon collections. In this work, we introduce a new and novel type of ionizing particle detector based on phonon collection. Helium ion radiation treats tumors with better precision. There are nine known isotopes of helium, but only helium-3 and helium-4 are stable. Helium-4 is formed in fusion reactor technology and in enormous quantities during Big Bang nucleo-synthesis. In this study, we introduce a technique for helium-4 ion detection (sensing) based on the innovative properties of the new composite materials known as phononic crystals (PnCs). PnCs can provide an easy and cheap technique for ion detection compared with conventional methods. PnC structures commonly consist of a periodic array of two or more materials with different elastic properties. The two materials are polymethyl-methacrylate and polyethylene polymers. The calculations showed that the energies lost to target phonons are maximized at 1 keV helium-4 ion energy. There is a correlation between the total phonon energies and the transmittance of PnC structures. The maximum transmission for phonons due to the passage of helium-4 ions was found in the case of making polyethylene as a first layer in the PnC structure. Therefore, the concept of ion detection based on PnC structure is achievable.
Ionizing particle detection based on phononic crystals
Energy Technology Data Exchange (ETDEWEB)
Aly, Arafa H., E-mail: arafa16@yahoo.com, E-mail: arafa.hussien@science.bsu.edu.eg; Mehaney, Ahmed; Eissa, Mostafa F. [Physics Department, Faculty of Science, Beni-Suef University, Beni-Suef (Egypt)
2015-08-14
Most conventional radiation detectors are based on electronic or photon collections. In this work, we introduce a new and novel type of ionizing particle detector based on phonon collection. Helium ion radiation treats tumors with better precision. There are nine known isotopes of helium, but only helium-3 and helium-4 are stable. Helium-4 is formed in fusion reactor technology and in enormous quantities during Big Bang nucleo-synthesis. In this study, we introduce a technique for helium-4 ion detection (sensing) based on the innovative properties of the new composite materials known as phononic crystals (PnCs). PnCs can provide an easy and cheap technique for ion detection compared with conventional methods. PnC structures commonly consist of a periodic array of two or more materials with different elastic properties. The two materials are polymethyl-methacrylate and polyethylene polymers. The calculations showed that the energies lost to target phonons are maximized at 1 keV helium-4 ion energy. There is a correlation between the total phonon energies and the transmittance of PnC structures. The maximum transmission for phonons due to the passage of helium-4 ions was found in the case of making polyethylene as a first layer in the PnC structure. Therefore, the concept of ion detection based on PnC structure is achievable.
Coherent phonons in carbon based nanostructures
Sanders, G. D.; Nugraha, A. R. T.; Sato, K.; Kim, J.-H.; Lim, Y.-S.; Kono, J.; Saito, R.; Stanton, C. J.
2014-06-01
We have developed a theory for the generation and detection of coherent phonons in carbon based nanotstructures such as single walled nanotubes (SWNTs), graphene, and graphene nanoribbons. Coherent phonons are generated via the deformation potential electron/hole-phonon interaction with ultrafast photo-excited carriers. They modulate the reflectance or absorption of an optical probe pules on a THz time scale and might be useful for optical modulators. In our theory the electronic states are treated in a third nearest neighbor extended tight binding formalism which gives a good description of the states over the entire Brillouin zone while the phonon states are treated using valence force field models which include bond stretching, in-plane and out-of-plane bond bending, and bond twisting interactions up to fourth neighbor distances. We compare our theory to experiments for the low frequency radial breathing mode (RBM) in micelle suspended single-walled nanotubes (SWNTs). The analysis of such data provides a wealth of information on the dynamics and interplay of photons, phonons and electrons in these carbon based nanostructures.
Phonon tunneling through a double barrier system
Energy Technology Data Exchange (ETDEWEB)
Villegas, Diosdado [Departamento de Física, Universidad Central “Marta Abreu” de Las Villas, CP 54830, Santa Clara, Villa Clara (Cuba); Instituto de Física, Universidad Autónoma de Puebla, 18 Sur y San Claudio, Edif. 110A, Ciudad Universitaria, 72570 Puebla (Mexico); León-Pérez, Fernando de [Centro Universitario de la Defensa de Zaragoza, Ctra. de Huesca s/n, E-50090 Zaragoza (Spain); Pérez-Álvarez, R. [Universidad Autónoma del Estado de Morelos, Av. Universidad 1001, CP 62209 Cuernavaca (Mexico); Arriaga, J., E-mail: arriaga@ifuap.buap.mx [Instituto de Física, Universidad Autónoma de Puebla, 18 Sur y San Claudio, Edif. 110A, Ciudad Universitaria, 72570 Puebla (Mexico)
2015-04-15
The tunneling of optical and acoustic phonons at normal incidence on a double-barrier is studied in this paper. Transmission coefficients and resonance conditions are derived theoretically under the assumption that the long-wavelength approximation is valid. It is shown that the behavior of the transmission coefficients for the symmetric double barrier has a Lorentzian form close to resonant frequencies and that Breit–Wigner's formula have a general validity in one-dimensional phonon tunneling. Authors also study the so-called generalized Hartman effect in the tunneling of long-wavelength phonons and show that this effect is a numerical artifact resulting from taking the opaque limit before exploring the variation with a finite barrier width. This study could be useful for the design of acoustic devices.
Phonon heat transport in gallium arsenide
Indian Academy of Sciences (India)
Richa Saini; Vinod Ashokan; B D Indu; R Kumar
2012-03-01
The lifetimes of quantum excitations are directly related to the electron and phonon energy linewidths of a particular scattering event. Using the versatile double time thermodynamic Green’s function approach based on many-body theory, an ab-initio formulation of relaxation times of various contributing processes has been investigated with newer understanding in terms of the linewidths of electrons and phonons. The energy linewidth is found to be an extremely sensitive quantity in the transport phenomena of crystalline solids as a collection of large number of scattering processes, namely, boundary scattering, impurity scattering, multiphonon scattering, interference scattering, electron–phonon processes and resonance scattering. The lattice thermal conductivities of three samples of GaAs have been analysed on the basis of modiﬁed Callaway model and a fairly good agreement between theory and experimental observations has been reported.
Toward quantitative modeling of silicon phononic thermocrystals
Energy Technology Data Exchange (ETDEWEB)
Lacatena, V. [STMicroelectronics, 850, rue Jean Monnet, F-38926 Crolles (France); IEMN UMR CNRS 8520, Institut d' Electronique, de Microélectronique et de Nanotechnologie, Avenue Poincaré, F-59652 Villeneuve d' Ascq (France); Haras, M.; Robillard, J.-F., E-mail: jean-francois.robillard@isen.iemn.univ-lille1.fr; Dubois, E. [IEMN UMR CNRS 8520, Institut d' Electronique, de Microélectronique et de Nanotechnologie, Avenue Poincaré, F-59652 Villeneuve d' Ascq (France); Monfray, S.; Skotnicki, T. [STMicroelectronics, 850, rue Jean Monnet, F-38926 Crolles (France)
2015-03-16
The wealth of technological patterning technologies of deca-nanometer resolution brings opportunities to artificially modulate thermal transport properties. A promising example is given by the recent concepts of 'thermocrystals' or 'nanophononic crystals' that introduce regular nano-scale inclusions using a pitch scale in between the thermal phonons mean free path and the electron mean free path. In such structures, the lattice thermal conductivity is reduced down to two orders of magnitude with respect to its bulk value. Beyond the promise held by these materials to overcome the well-known “electron crystal-phonon glass” dilemma faced in thermoelectrics, the quantitative prediction of their thermal conductivity poses a challenge. This work paves the way toward understanding and designing silicon nanophononic membranes by means of molecular dynamics simulation. Several systems are studied in order to distinguish the shape contribution from bulk, ultra-thin membranes (8 to 15 nm), 2D phononic crystals, and finally 2D phononic membranes. After having discussed the equilibrium properties of these structures from 300 K to 400 K, the Green-Kubo methodology is used to quantify the thermal conductivity. The results account for several experimental trends and models. It is confirmed that the thin-film geometry as well as the phononic structure act towards a reduction of the thermal conductivity. The further decrease in the phononic engineered membrane clearly demonstrates that both phenomena are cumulative. Finally, limitations of the model and further perspectives are discussed.
Theory of coherent phonons in carbon nanotubes and graphene nanoribbons
Sanders, G. D.; Stanton, C. J.; Nugraha, A. R. T.; Saito, R.
2013-03-01
We have performed theoretical studies on generating and detecting coherent radial breathing mode (RBM) phonons in single-walled carbon nanotubes and coherent radial breathing like mode (RBLM) phonons in graphene nanoribbons. A microscopic theory incorporating electronic states, phonon modes, optical matrix elements, and electron-phonon interaction matrix elements allows us to calculate the coherent phonon spectrum. The coherent phonon amplitudes satisfy a driven oscillator equation with a driving term that depends on photoexcited carrier density. We study the coherent phonon spectrum for nanotubes of different chirality and for armchair and zigzag graphene nanoribbons. We compare our results with a simpler, effective mass theory where we find reasonable agreement with the main features of our computed coherent phonon spectrum. Supported by NSF through grants OISE-0968405 and DMR-1105437 and MEXT through grant No. 20241023
A chip-integrated coherent photonic-phononic memory
Merklein, Moritz; Vu, Khu; Madden, Stephen J; Eggleton, Benjamin J
2016-01-01
Controlling and manipulating quanta of coherent acoustic vibrations - phonons - in integrated circuits has recently drawn a lot of attention, as phonons can function as unique links between radiofrequency and optical signals and access quantum regimes. It has been shown that radiofrequency signals can be controlled and stored via piezo-electrically actuated coherent phonons. Coherent phonons, however, can also be directly excited by optical photons through strong acousto-optic coupling in integrated circuits that guide photons as well as phonons. These hypersound phonons have similar wavelength as the exciting optical field but travel at a 5-orders of magnitude lower velocity. This allows the realization of a coherent optical buffer, a long time desired yet elusive device for on-chip optical signal processing. In this letter we demonstrate a coherent on-chip memory storing the entire coherent information carried by light, phase and amplitude, as acoustic phonons. The photonic-phononic memory provides GHz-band...
Murzin, Serguei P.; Balyakin, Valeriy B.
2017-02-01
A possibility of microstructuring the surface of silicon carbide ceramic by pulse-periodic laser treatment was determined for reducing the coefficient of friction under actual contact stress conditions that occur in elements of the rolling bearing in operation. Temperature rate conditions for the laser treatment with pulse duration in the millisecond range were found, which lead to a change in the surface microrelief of silicon carbide ceramic obtained by diamond grinding after hot isostatic pressing. The determination of the coefficient of sliding friction was conducted with using the ball-on-disk tribometer at normal loads, which corresponds to the values of contact stresses of (0.5-1)×109 Pa. When the load was increased to the upper limit of measuring range, the friction coefficient decrease after laser treatment was more than 30% compared to the initial structure. Significant reduction of friction in rolling bearings up to this level provides an opportunity to improve efficiency of various machines.
Ageev, E. I.; Andreeva, Ya M.; Karlagina, Yu Yu; Kolobov, Yu R.; Manokhin, S. S.; Odintsova, G. V.; Slobodov, A. A.; Veiko, V. P.
2017-04-01
A pulsed fiber laser with a wavelength of 1.06 µm was used to treat a commercial pure titanium surface in the air at intensities below the ablation threshold to provide oxide formation. Laser oxidation results are predicted by the chemical thermodynamic method and confirmed by experimental techniques (x-ray diffraction, energy dispersive x-ray spectroscopy). For the first time, the chemical thermodynamic method was used for determining the qualitative and quantitative phase-chemical composition of the compounds formed by a pulsed laser heating of commercial titanium in the air, and its applicability is proven. The simulation shows that multilayered composite film appears on a surface, the lower layers of which consist of Ti2O3 and TiO oxides with the addition of titanium nitride; and the thin upper layer consists of transparent titanium dioxide. Also, the chemical composition of films remains unchanged within a temperature range of 881–2000 K.
Phonon dispersion curves of CsCN
Indian Academy of Sciences (India)
N K Gaur; Preeti Singh; E G Rini; Jyotsna Galgale; R K Singh
2004-08-01
The motivation for the present work was gained from the recent publication on phonon dispersion curves (PDCs) of CsCN from the neutron scattering technique. We have applied the extended three-body force shell model (ETSM) by incorporating the effect of coupling between the translation modes and the orientation of cyanide molecules for the description of phonon dispersion curves of CsCN between the temperatures 195 and 295 K. Our results on PDCs in symmetric direction are in good agreement with the experimental data measured with inelastic neutron scattering technique.
Phonon-Josephson resonances in atomtronic circuits
Bidasyuk, Y. M.; Prikhodko, O. O.; Weyrauch, M.
2016-09-01
We study the resonant excitation of sound modes from Josephson oscillations in Bose-Einstein condensates. From the simulations for various setups using the Gross-Pitaevskii mean-field equations and Josephson equations we observe additional tunneling currents induced by resonant phonons. The proposed experiment may be used for spectroscopy of phonons as well as other low-energy collective excitations in Bose-Einstein condensates. We also argue that the observed effect may mask the observation of Shapiro resonances if not carefully controlled.
Timofeev, I. S.; Burdonskiy, I. N.; Goltsov, A. Yu; Leonov, A. G.; Makarov, K. N.; Yufa, V. N.
2016-09-01
The paper presents the analysis of interaction of the high-power laser pulse with multicomponent polycrystal rocks. Experiments were completed on a laser facility “Saturn” with intensity of 1010-1013 W/cm2. Structural analysis of the materials from the spall crater and from the plasma flame show significant differences. The article demonstrates experimental results of the spall formation moment depending on the thickness of the radiated target. The scale of damage to aluminium 6 pm thick foil at the rare side of the target is illustrated when it is hit by the andesite fragments from a spall crater.
Energy Technology Data Exchange (ETDEWEB)
Tuchina, E S; Petrov, P O; Kozina, K V; Tuchin, V V [N.G. Chernyshevsky Saratov State University, Saratov (Russian Federation); Ratto, F; Pini, R [Institute of Applied Physics ' Nello Carrara' , National Research Council, via Madonna del Piano 10 50019 Sesto Fiorentino (Italy); Centi, S [University of Florence, Dept. Experimental and Clinical Biomedical Sciences, viale Morgagni 50, 50134 Firenze (Italy)
2014-07-31
The effect of NIR laser radiation (808 nm) and gold nanorods on the cells of two strains of Staphylococcus aureus, one of them being methicillin-sensitive and the other being methicillinresistant, is studied. Nanorods having the dimensions 10 × 44 nm with the absorption maximum in the NIR spectral region, functionalised with human immunoglobulins IgA and IgG, are synthesised. It is shown that the use of nanoparticles in combination with NIR irradiation leads to killing up to 97% of the population of microorganisms. (laser biophotonics)
Selective coherent phonon-mode generation in single-wall carbon nanotubes
Nugraha, Ahmad R. T.; Hasdeo, Eddwi H.; Saito, Riichiro
2017-02-01
The pulse-train technique within ultrafast pump-probe spectroscopy is theoretically investigated to excite a specific coherent phonon mode while suppressing the other phonon modes generated in single-wall carbon nanotubes (SWNTs). In particular, we focus on the selectivity of the radial breathing mode (RBM) and the G-band for a given SWNT. We find that if the repetition period of the pulse train matches with the integer multiple of the RBM phonon period, the RBM amplitude can be maintained while the amplitudes of the other modes are suppressed. As for the G-band, when we apply a repetition period of a half-integer multiple of the RBM period, the RBM can be suppressed because of destructive interference, while the G-band still survives. It is also possible to keep the G-band and suppress the RBM by applying a repetition period that matches with the integer multiple of the G-band phonon period. However, in this case we have to use a large number of laser pulses having a property of “magic ratio” of the G-band and RBM periods.
Band structure characteristics of T-square fractal phononic crystals
Institute of Scientific and Technical Information of China (English)
Liu Xiao-Jian; Fan You-Hua
2013-01-01
The T-square fractal two-dimensional phononic crystal model is presented in this article.A comprehensive study is performed for the Bragg scattering and locally resonant fractal phononic crystal.We find that the band structures of the fractal and non-fractal phononic crystals at the same filling ratio are quite different through using the finite element method.The fractal design has an important impact on the band structures of the two-dimensional phononic crystals.
Optical phonons in Ge quantum dots obtained on Si(111)
Talochkin, A B
2002-01-01
The light combination scattering on the optical phonons in the Ge quantum dots, obtained on the Si surface of the (111) orientation through the molecular-beam epitaxy, is studied. The series of lines, connected with the phonon spectrum quantization, was observed. It is shown, that the phonon modes frequencies are well described by the elastic properties and dispersion of the voluminous Ge optical phonons. The value of the Ge quantum dots deformation is determined
Yi, Kyung-Soo; Kim, Hye-Jung
2017-02-01
We investigate spectral behavior of phonon spectral functions in an interacting multi-component hot carrier plasma. Spectral analysis of various phonon spectral functions is performed considering carrier-phonon channels of polar and nonpolar optical phonons, acoustic deformation-potential, and piezoelectric Coulomb couplings. Effects of phonon self-energy corrections are examined at finite temperature within a random phase approximation extended to include the effects of dynamic screening, plasmon-phonon coupling, and local-field corrections of the plasma species. We provide numerical data for the case of a photo-generated electron-hole plasma formed in a wurtzite GaN. Our result shows the clear significance of the multiplicity of the plasma species in the phonon spectral functions of a multi-component plasma giving rise to a variety of spectral behaviors of carrier-phonon coupled collective modes. A useful sum rule on the plasma-species-resolved dielectric functions is also found.
Manipulating Heat Flow through 3 Dimensional Nanoscale Phononic Crystal Structure
2014-06-02
SUBJECT TERMS phonon transport , Thermoelectric, nano structures, nano photonics 16. SECURITY CLASSIFICATION OF: 17. LIMITATION OF ABSTRACT Same as...conductivity is also studied. 15. SUBJECT TERMS phonon transport , Thermoelectric, nano structures, nano photonics 16. SECURITY CLASSIFICATION OF: 17...but not yet published L-N Yang, J Chen, N Yang, and B Li, Manipulating Graphene Thermal Conductivity by Phononic
Wang, Yan; Lu, Zexi; Ruan, Xiulin
2016-06-01
The effect of phonon-electron (p-e) scattering on lattice thermal conductivity is investigated for Cu, Ag, Au, Al, Pt, and Ni. We evaluate both phonon-phonon (p-p) and p-e scattering rates from first principles and calculate the lattice thermal conductivity (κL). It is found that p-e scattering plays an important role in determining the κL of Pt and Ni at room temperature, while it has negligible effect on the κL of Cu, Ag, Au, and Al. Specifically, the room temperature κLs of Cu, Ag, Au, and Al predicted from density-functional theory calculations with the local density approximation are 16.9, 5.2, 2.6, and 5.8 W/m K, respectively, when only p-p scattering is considered, while it is almost unchanged when p-e scattering is also taken into account. However, the κL of Pt and Ni is reduced from 7.1 and 33.2 W/m K to 5.8 and 23.2 W/m K by p-e scattering. Even though Al has quite high electron-phonon coupling constant, a quantity that characterizes the rate of heat transfer from hot electrons to cold phonons in the two-temperature model, p-e scattering is not effective in reducing κL owing to the relatively low p-e scattering rates in Al. The difference in the strength of p-e scattering in different metals can be qualitatively understood by checking the amount of electron density of states that is overlapped with the Fermi window. Moreover, κL is found to be comparable to the electronic thermal conductivity in Ni.
``Forbidden'' phonon in the iron chalcogenide series
Fobes, David M.; Zaliznyak, Igor A.; Xu, Zhijun; Gu, Genda; Tranquada, John M.
2015-03-01
Recently, we uncovered evidence for the formation of a bond-order wave (BOW) leading to ferro-orbital order at low temperature, acting to stabilize the bicollinear AFM order, in the iron-rich parent compound, Fe1+yTe. Investigating the inelastic spectra centered near (100) in Fe1+yTe, a signature peak for the BOW formation in the monoclinic phase, we observed an acoustic phonon dispersion in both tetragonal and monoclinic phases. While a structural Bragg peak accompanies the mode in the monoclinic phase, in the tetragonal phase Bragg scattering at this Q is forbidden by symmetry, and we observed no elastic peak. This phonon mode was also observed in superconducting FeTe0.6Se0.4, where structural and magnetic transitions are suppressed. LDA frozen phonon calculations suggested that this mode could result from a spin imbalance between neighboring Fe atoms, but polarized neutron measurements revealed no additional magnetic scattering. We propose that this ``forbidden'' phonon mode may originate from dynamically broken symmetry, perhaps related to the strong dynamic spin correlations in these materials. Work at BNL was supported by BES, US DOE, under Contract No. DE-AC02-98CH10886. Research at ORNL's HFIR and SNS sponsored by Scientific User Facilities Division, BES, US DOE. We acknowledge the support of NIST, in providing neutron research facilities.
Resonant tunneling in a pulsed phonon field
DEFF Research Database (Denmark)
Kral, P.; Jauho, Antti-Pekka
1999-01-01
We theoretically investigate resonant tunneling through a single level assisted by short LO phonon pulses. The analysis is based on the recently developed nonequilibrium linked-cluster expansion [P. Kral, Phys. Rev. B 56, 7293 (1997)], extended in this work to transient situations, The nonequilib...
Hyperbolic phonon polaritons in hexagonal boron nitride
Dai, Siyuan
2015-03-01
Uniaxial materials whose axial and tangential permittivities have opposite signs are referred to as indefinite or hyperbolic media. While hyperbolic responses are normally achieved with metamaterials, hexagonal boron nitride (hBN) naturally possesses this property due to the anisotropic phonons in the mid-infrared. Using scattering-type scanning near-field optical microscopy, we studied polaritonic phenomena in hBN. We performed infrared nano-imaging of highly confined and low-loss hyperbolic phonon polaritons in hBN. The polariton wavelength was shown to be governed by the hBN thickness according to a linear law persisting down to few atomic layers [Science, 343, 1125-1129 (2014)]. Additionally, we carried out the modification of hyperbolic response in heterostructures comprised of a mononlayer graphene deposited on hBN. Electrostatic gating of the top graphene layer allows for the modification of wavelength and intensity of hyperbolic phonon polaritons in bulk hBN. The physics of the modification originates from the plasmon-phonon coupling in the hyperbolic medium. Furthermore, we demonstrated the ``hyperlens'' for subdiffractional imaging and focusing using a slab of hBN.
Phonon scattering in graphene over substrate steps
DEFF Research Database (Denmark)
Sevincli, Haldun; Brandbyge, Mads
2014-01-01
We calculate the effect on phonon transport of substrate-induced bends in graphene. We consider bending induced by an abrupt kink in the substrate, and provide results for different step-heights and substrate interaction strengths. We find that individual substrate steps reduce thermal conductance...
Parity-Time Synthetic Phononic Media
DEFF Research Database (Denmark)
Christensen, Johan; Willatzen, Morten; Velasco, V. R.
2016-01-01
, are achieved through electrically biased piezoelectric semiconductors. We study first how wave attenuation and amplification can be tuned, and when combined, can give rise to a phononic PT synthetic media with unidirectional suppressed reflectance, a feature directly applicable to evading sonar detection....
Synthetic thermoelectric materials comprising phononic crystals
El-Kady, Ihab F; Olsson, Roy H; Hopkins, Patrick; Reinke, Charles; Kim, Bongsang
2013-08-13
Synthetic thermoelectric materials comprising phononic crystals can simultaneously have a large Seebeck coefficient, high electrical conductivity, and low thermal conductivity. Such synthetic thermoelectric materials can enable improved thermoelectric devices, such as thermoelectric generators and coolers, with improved performance. Such synthetic thermoelectric materials and devices can be fabricated using techniques that are compatible with standard microelectronics.
Uniaxial strain-induced Kohn anomaly and electron-phonon coupling in acoustic phonons of graphene
Cifuentes-Quintal, M. E.; de la Peña-Seaman, O.; Heid, R.; de Coss, R.; Bohnen, K.-P.
2016-08-01
Recent advances in strain engineering at the nanoscale have shown the feasibility to modulate the properties of graphene. Although the electron-phonon (e-ph) coupling and Kohn anomalies in graphene define the phonon branches contributing to the resonance Raman scattering and are relevant to the electronic and thermal transport as a scattering source, the evolution of the e-ph coupling as a function of strain has been less studied. In this work, the Kohn anomalies and the e-ph coupling in uniaxially strained graphene along armchair and zigzag directions were studied by means of density functional perturbation theory calculations. In addition to the phonon anomaly at the transversal optical (TO) phonon branch in the K point for pristine graphene, we found that uniaxial strain induces a discontinuity in the frequency derivative of the longitudinal acoustic phonon branch. This behavior corresponds to the emergence of a Kohn anomaly, as a consequence of a strain-enhanced e-ph coupling. Thus, the present results for uniaxially strained graphene contrast with the commonly assumed view that the e-ph coupling around the K point is only present in the TO phonon branch.
Unified theory of electron-phonon renormalization and phonon-assisted optical absorption.
Patrick, Christopher E; Giustino, Feliciano
2014-09-10
We present a theory of electronic excitation energies and optical absorption spectra which incorporates energy-level renormalization and phonon-assisted optical absorption within a unified framework. Using time-independent perturbation theory we show how the standard approaches for studying vibronic effects in molecules and those for addressing electron-phonon interactions in solids correspond to slightly different choices for the non-interacting Hamiltonian. Our present approach naturally leads to the Allen-Heine theory of temperature-dependent energy levels, the Franck-Condon principle, the Herzberg-Teller effect and to phonon-assisted optical absorption in indirect band gap materials. In addition, our theory predicts sub-gap phonon-assisted optical absorption in direct gap materials, as well as an exponential edge which we tentatively assign to the Urbach tail. We also consider a semiclassical approach to the calculation of optical absorption spectra which simultaneously captures energy-level renormalization and phonon-assisted transitions and is especially suited to first-principles electronic structure calculations. We demonstrate this approach by calculating the phonon-assisted optical absorption spectrum of bulk silicon.
Phonon-assisted intersubband transitions in wurtzite GaN/InxGa1-xN quantum wells
Institute of Scientific and Technical Information of China (English)
Zhu Jun; Ban Shi-Liang; Ha Si-Hua
2012-01-01
A detailed numerical calculation on the phonon-assisted intersubband transition rates of electrons in wurtzite GaN/InxGa1-xN quantum wells is presented. The quantum-confined Stark effect,induced by the built-in electric field,and the ternary mixed crystal effect are considered.The electron states are obtained by iteratively solving the coupled Schr(o)dinger and Poisson equations.The dispersion properties of each type of phonon modes are considered in the derivation of Fermi's golden rule to evaluate the transition rates.It is indicated that the interface and halfspace phonon scattering play an important role in the process of 1-2 radiative transition.The transition rate is also greatly reduced by the built-in electric field.This work can be helpful for the structural design and simulation of new semiconductor lasers.
The phonon and thermal properties of a ladder nanostructure
Directory of Open Access Journals (Sweden)
M Mardaani
2011-12-01
Full Text Available In this paper, we study the phonon thermal properties of a ladder nanostructure in harmonic approximation. We present a model consisting of two infinite chains with different masses. Then, we investigate the effect of different masses on the phonon spectrum. Moreover, as a specific case, in the absence of the second neighbor interaction, we calculate the phonon density of states/modes. Finally, we consider the thermal conductivity of the system. The results show that the phonon spectrum shifts down to the lower frequencies by increasing the masses. Furthermore, a frequency gap appears in the phonon spectrum. By increasing the springs constants, the thermal conductance decreases.
Molecular dynamics study of phonon screening in graphene
Javvaji, Brahmanandam; Roy Mahapatra, D.; Raha, S.
2014-04-01
Phonon interaction with electrons or phonons or with structural defects result in a phonon mode conversion. The mode conversion is governed by the frequency wave-vector dispersion relation. The control over phonon mode or the screening of phonon in graphene is studied using the propagation of amplitude modulated phonon wave-packet. Control over phonon properties like frequency and velocity opens up several wave guiding, energy transport and thermo-electric applications of graphene. One way to achieve this control is with the introduction of nano-structured scattering in the phonon path. Atomistic model of thermal energy transport is developed which is applicable to devices consisting of source, channel and drain parts. Longitudinal acoustic phononmode is excited fromone end of the device. Molecular dynamics based time integration is adopted for the propagation of excited phonon to the other end of the device. The amount of energy transfer is estimated from the relative change of kinetic energy. Increase in the phonon frequency decreases the kinetic energy transmission linearly in the frequency band of interest. Further reduction in transmission is observed with the tuning of channel height of the device by increasing the boundary scattering. Phonon mode selective transmission control have potential application in thermal insulation or thermo-electric application or photo-thermal amplification.
Phonon density of states in nanocrystalline 57Fe
Indian Academy of Sciences (India)
Ranber Singh; S Prakash; R Meyer; P Entel
2003-03-01
The Born–von Karman model is used to calculate phonon density of states (DOS) of nanocrystalline bcc Fe. It is found that there is an anisotropic stiffening in the interatomic force constants and hence there is shrinking in the nearest-neighbour distances in the nanophase. This leads to additional vibrational modes above the bulk phonons near the bottom of the phonon band. It is found that the high energy phonon modes of nanophase Fe are the surface modes. The calculated phonon DOS closely agree with the experimental data except a peak at 37 meV. The calculated phonon dispersion relations are also compared with those of the bulk phonons and anomalous behaviour is discussed in detail. The speciﬁc heat in nanophase enhances as compared to bulk phase at low temperatures and the calculated Debye temperature agrees with the experimental results. It is predicted that the nanocrystalline Fe may consist of about 14 GPa pressure.
Mante, Pierre-Adrien; Stoumpos, Constantinos C.; Kanatzidis, Mercouri G.; Yartsev, Arkady
2017-01-01
Despite the great amount of attention CH3NH3PbI3 has received for its solar cell application, intrinsic properties of this material are still largely unknown. Mobility of charges is a quintessential property in this aspect; however, there is still no clear understanding of electron transport, as reported values span over three orders of magnitude. Here we develop a method to measure the electron and hole deformation potentials using coherent acoustic phonons generated by femtosecond laser pulses. We apply this method to characterize a CH3NH3PbI3 single crystal. We measure the acoustic phonon properties and characterize electron-acoustic phonon scattering. Then, using the deformation potential theory, we calculate the carrier intrinsic mobility and compare it to the reported experimental and theoretical values. Our results reveal high electron and hole mobilities of 2,800 and 9,400 cm2 V−1 s−1, respectively. Comparison with literature values of mobility demonstrates the potential role played by polarons in charge transport in CH3NH3PbI3. PMID:28176755
Mante, Pierre-Adrien; Stoumpos, Constantinos C.; Kanatzidis, Mercouri G.; Yartsev, Arkady
2017-02-01
Despite the great amount of attention CH3NH3PbI3 has received for its solar cell application, intrinsic properties of this material are still largely unknown. Mobility of charges is a quintessential property in this aspect; however, there is still no clear understanding of electron transport, as reported values span over three orders of magnitude. Here we develop a method to measure the electron and hole deformation potentials using coherent acoustic phonons generated by femtosecond laser pulses. We apply this method to characterize a CH3NH3PbI3 single crystal. We measure the acoustic phonon properties and characterize electron-acoustic phonon scattering. Then, using the deformation potential theory, we calculate the carrier intrinsic mobility and compare it to the reported experimental and theoretical values. Our results reveal high electron and hole mobilities of 2,800 and 9,400 cm2 V-1 s-1, respectively. Comparison with literature values of mobility demonstrates the potential role played by polarons in charge transport in CH3NH3PbI3.
Watanabe, Yohei; Hino, Ken-ichi; Hase, Muneaki; Maeshima, Nobuya
2017-01-01
We examine generation dynamics of coherent phonons in both polar and nonpolar semiconductors, such as GaAs and Si, based on a polaronic-quasiparticle (PQ) model. In this model, the PQ operator is composed of two kinds of operators: one is a quasiboson operator, defined as a linear combination of a set of pairs of electron operators, and the other is a longitudinal optical (LO) phonon operator. In particular, the problem of transient and nonlinear Fano resonance (FR) is tackled, where the vestige of this quantum interference effect was observed exclusively in lightly n -doped Si immediately after carriers were excited by an ultrashort pulse laser [M. Hase et al., Nature (London) 426, 51 (2003), 10.1038/nature02044], although not observed yet in GaAs. The PQ model enables us to show straightforwardly that the phonon energy state is embedded in continuum states formed by a set of adiabatic eigenstates of the quasiboson; this energy configuration is a necessary condition of the manifestation of the transient FR in the present optically nonlinear system. Numerical calculations are done for photoemission spectra relevant to the retarded longitudinal dielectric function of transient photoexcited states and for power spectra relevant to the LO-phonon displacement function of time. The photoemission spectra show that in undoped Si, an asymmetric spectral profile characteristic of FR comes into existence immediately after the instantaneous carrier excitation to fade out gradually, whereas in undoped GaAs, no asymmetry in spectra appears in the whole temporal region. The similar results are also obtained in the power spectra. These results are in harmony with the reported experimental results. It is found that the obtained difference in spectral profile between undoped Si and GaAs is attributed to a phase factor of an effective interaction between the LO phonon and the quasiboson. More detailed discussion of the FR dynamics is made in the text.
Dynamically coupled plasmon-phonon modes in GaP: An indirect-gap polar semiconductor
Ishioka, Kunie; Brixius, Kristina; Höfer, Ulrich; Rustagi, Avinash; Thatcher, Evan M.; Stanton, Christopher J.; Petek, Hrvoje
2015-11-01
The ultrafast coupling dynamics of coherent optical phonons and the photoexcited electron-hole plasma in the indirect gap semiconductor GaP are investigated by experiment and theory. For below-gap excitation and probing by 800-nm light, only the bare longitudinal optical (LO) phonons are observed. For above-gap excitation with 400-nm light, the photoexcitation creates a high density, nonequilibrium e -h plasma, which introduces an additional, faster decaying oscillation due to an LO phonon-plasmon coupled (LOPC) mode. The LOPC mode frequency exhibits very similar behavior for both n - and p -doped GaP, downshifting from the LO to the transverse optical (TO) phonon frequency limits with increasing photoexcited carrier density. We assign the LOPC mode to the LO phonons coupled with the photoexcited multicomponent plasma. For the 400-nm excitation, the majority of the photoexcited electrons are scattered from the Γ valley into the satellite X valley, while the light and spin-split holes are scattered into the heavy hole band, within 30 fs. The resulting mixed plasma is strongly damped, leading to the LOPC frequency appearing in the reststrahlen gap. Due to the large effective masses of the X electrons and heavy holes, the coupled mode appears most distinctly at carrier densities ≳5 ×1018cm-3 . We perform theoretical calculations of the nuclear motions and the electronic polarizations following an excitation with an ultrashort optical pulse to obtain the transient reflectivity responses of the coupled modes. We find that, while the longitudinal diffusion of photoexcited carriers is insignificant, the lateral inhomogeneity of the photoexcited carriers due to the laser intensity profile should be taken into account to reproduce the major features of the observed coupled mode dynamics.
Confocal Raman depth-scanning spectroscopic study of phonon-plasmon modes in GaN epilayers
Strelchuk, V. V.; Bryksa, V. P.; Avramenko, K. A.; Valakh, M. Ya.; Belyaev, A. E.; Mazur, Yu. I.; Ware, M. E.; DeCuir, E. A.; Salamo, G. J.
2011-06-01
Coupled longitudinal-optical (LO)-phonon-plasmon excitations were studied using confocal micro-Raman spectroscopy. The high-quality Si-doped GaN epilayers were grown in a Gunn diode structure on (0001) sapphire substrates by plasma assisted molecular beam epitaxy. Depth-profiled Raman spectra exhibit a spatial variation of both low, ω-, and high, ω+, frequency coupled phonon-plasmon modes (CPPMs) in the n-GaN layers. To describe the features of the CPPMs in the Raman spectra a self-consistent model that includes both the electro-optic and deformation-potential as well as charge-density fluctuation mechanisms as important processes for light scattering in n-GaN has been proposed. An agreement between the theoretical and experimental line shapes of the Raman spectra is obtained. From the best line-shape fitting of the CPPMs the depth profiles of the plasmon and phonon damping, plasmon frequency, free carrier concentrations, and electron mobility as well as the contributions of the electron-phonon interaction and charge density fluctuations to the Raman cross section in the GaN layers are determined. It is found that these depth profiles exhibit considerable nonuniformity and change at different laser pump-power excitations. Despite the high electron concentration in the n+-GaN layers, a strong peak of the unscreened A1(LO) phonon is also observed. A possible origin for the appearance of this mode is discussed.
Generating Coherent Phonons and Spin Excitations with Ultrafast Light Pulses
Merlin, Roberto
2006-03-01
Recent work on the generation of coherent low-lying excitations by ultrafast laser pulses will be reviewed, emphasizing the microscopic mechanisms of light-matter interaction. The topics covered include long-lived phonons in ZnO [C. Aku-Leh, J. Zhao, R. Merlin, J. Men'endez and M. Cardona, Phys. Rev.B 71, 205211 (2005)], squeezed magnons [J. Zhao, A. V. Bragas, D. J. Lockwood and R. Merlin, Phys. Rev. Lett. 93, 107203 (2004)], spin- and charge-density fluctuations [J. M. Bao et al., Phys. Rev. Lett. 92, 236601 (2004)] and cyclotron resonance [J. K. Wahlstrand, D. M. Wang, P. Jacobs, J. M. Bao, R. Merlin, K. W. West and L. N. Pfeiffer, AIP Conference Proceedings 772 (2005), p. 1313] in GaAs quantum wells. In addition, unpublished results on surface -avoiding phonons in GaAs-AlAs superlattices [M. Trigo et al., unpublished] and magnons in ferromagnetic Ga1-xMnxAs [D. M. Wang et al., unpublished] will be discussed. It will also be shown that frequencies can be measured using pump-probe techniques with a precision comparable to that of Brillouin scattering. It is now widely accepted that stimulated Raman scattering (SRS) is (often but not always) the mechanism responsible for the coherent coupling. Results will be presented showing that SRS is described by two separate tensors, one of which accounts for the excitation-induced modulation of the susceptibility, and the other one for the dependence of the amplitude of the oscillation on the light intensity [T. E. Stevens, J. Kuhl and R. Merlin, Phys. Rev. B 65, 144304 (2002)]. These tensors have the same real component, associated with impulsive coherent generation, but different imaginary parts. If the imaginary term dominates, that is, for strongly absorbing substances, the mechanism for two-band processes becomes displacive in nature, as in the DECP (displacive excitation of coherent phonons) model. It will be argued that DECP is not a separate mechanism, but a particular case of SRS. In the final part of the talk, an
Ab initio determination of effective electron-phonon coupling factor in copper
Ji, Pengfei; Zhang, Yuwen
2016-04-01
The electron temperature Te dependent electron density of states g (ε), Fermi-Dirac distribution f (ε), and electron-phonon spectral function α2 F (Ω) are computed as prerequisites before achieving effective electron-phonon coupling factor Ge-ph. The obtained Ge-ph is implemented into a molecular dynamics (MD) and two-temperature model (TTM) coupled simulation of femtosecond laser heating. By monitoring temperature evolutions of electron and lattice subsystems, the result utilizing Ge-ph from ab initio calculation shows a faster decrease of Te and increase of Tl than those using Ge-ph from phenomenological treatment. The approach of calculating Ge-ph and its implementation into MD-TTM simulation is applicable to other metals.
Ab initio determination of effective electron-phonon coupling factor in copper
Ji, Pengfei
2016-01-01
The electron temperature T_e dependent electron density of states g({\\epsilon}), Fermi-Dirac distribution f({\\epsilon}), and electron-phonon spectral function {\\alpha}^2 F({\\Omega}) are computed as prerequisites before achieving effective electron-phonon coupling factor. The obtained is implemented into a molecular dynamics (MD) and two-temperature model (TTM) coupled simulation of femtosecond laser heating. By monitoring temperature evolutions of electron and lattice subsystems, the result utilizing G_(e-ph) from ab initio calculation, shows a faster decrease of T_e and increase of T_l than those using G_(e-ph) from phenomenological treatment. The approach of calculating G_(e-ph) and its implementation into MD-TTM simulation is applicable to other metals.
Ultrafast spectroscopy of coherent phonon in carbon nanotubes using sub-5-fs visible pulses
Energy Technology Data Exchange (ETDEWEB)
Kobayashi, Takayoshi [Advanced Ultrafast Laser Research Center, The University of Electro-Communications, 1-5-1 Chofugaoka, Chofu, Tokyo, 182-8585 (Japan); JST, CREST, 5 Sanbancho, Chiyoda-ku, Tokyo 102-0075 Japan (Japan); Department of Electrophysics, National Chiao Tung University, Hsinchu 30010, Taiwan (China); Institute of Laser Engineering, Osaka University, 2-6 Yamada-oka, Suita, Osaka 565-0871, Japan kobayashi@ils.uec.ac.jp (Japan)
2016-02-01
In the last two decades, nano materials are attracting many scientists’ interest for both basic and application viewpoints. In order to understand the properties of nano systems it is needed to understand the dynamic properties which control the specific properties of the systems. All the primary processes in nano systems are taking place in femtosecond regime. Our group has been able to stably generate visible to near-infrared sub-5-fs laser pulses using a noncollinear optical parametric amplifier (NOPA) by the combination of various novel techniques including non-collinear optical parametric amplifier, pulse compression by a prism pair and grating pair. We apply the sub-5-fs pulses to study real-time coherent phonon in a one-dimensional system of carbon nanotubes. We determine exciton-phonon coupling mechanisms by observing the breathing mode in semiconducting carbon nanotubes and show the effect of electronic transition affected by the vibrational mode.
Magnons and Phonons Optically Driven out of Local Equilibrium in a Magnetic Insulator
An, Kyongmo; Olsson, Kevin S.; Weathers, Annie; Sullivan, Sean; Chen, Xi; Li, Xiang; Marshall, Luke G.; Ma, Xin; Klimovich, Nikita; Zhou, Jianshi; Shi, Li; Li, Xiaoqin
2016-09-01
The coupling and possible nonequilibrium between magnons and other energy carriers have been used to explain several recently discovered thermally driven spin transport and energy conversion phenomena. Here, we report experiments in which local nonequilibrium between magnons and phonons in a single crystalline bulk magnetic insulator, Y3Fe5O12 , has been created optically within a focused laser spot and probed directly via micro-Brillouin light scattering. Through analyzing the deviation in the magnon number density from the local equilibrium value, we obtain the diffusion length of thermal magnons. By explicitly establishing and observing local nonequilibrium between magnons and phonons, our studies represent an important step toward a quantitative understanding of various spin-heat coupling phenomena.
Indian Academy of Sciences (India)
R K Khanna; R C Chouhan
2003-10-01
A somewhat more general analysis for solving spatial propagation characteristics of intense Gaussian beam is presented and applied to the laser beam propagation in step-index proﬁle as well as parabolic proﬁle dielectric ﬁbers with Kerr non-linearity. Considering self-action due to saturating and non-saturating non-linearity in the refractive index, a general theory has been developed without any kind of power series expansion for the dielectric constant as is usually done in other theories that make use of paraxial approximation. Result of the steady state self-focusing analysis indicates that the Kerr non-linearity acts as a perturbation on the radial inhomogeneity due to ﬁber geometry. Analysis indicates that the paraxial rays and peripheral rays focus at different points, indicating aberration effect. Calculated critical power matches with the experimentally reported result.
Energy Technology Data Exchange (ETDEWEB)
Yu, Jen-Kan; Mitrovic, Slobodan; Heath, James R.
2016-08-16
A nanomesh phononic structure includes: a sheet including a first material, the sheet having a plurality of phononic-sized features spaced apart at a phononic pitch, the phononic pitch being smaller than or equal to twice a maximum phonon mean free path of the first material and the phononic size being smaller than or equal to the maximum phonon mean free path of the first material.
Hu, Huayu
2015-01-01
Nonperturbative calculation of QED processes participated by a strong electromagnetic field, especially provided by strong laser facilities at present and in the near future, generally resorts to the Furry picture with the usage of analytical solutions of the particle dynamical equation, such as the Klein-Gordon equation and Dirac equation. However only for limited field configurations such as a plane-wave field could the equations be solved analytically. Studies have shown significant interests in QED processes in a strong field composed of two counter-propagating laser waves, but the exact solutions in such a field is out of reach. In this paper, inspired by the observation of the structure of the solutions in a plane-wave field, we develop a new method and obtain the analytical solution for the Klein-Gordon equation and equivalently the action function of the solution for the Dirac equation in this field, under a largest dynamical parameter condition that there exists an inertial frame in which the particl...
Energy Technology Data Exchange (ETDEWEB)
Giri, Ashutosh; Gaskins, John T.; Foley, Brian M.; Cheaito, Ramez; Hopkins, Patrick E., E-mail: phopkins@virginia.edu [Department of Mechanical and Aerospace Engineering, University of Virginia, Charlottesville, Virginia 22904 (United States)
2015-01-28
The electronic transport properties of metals with weak electron-phonon coupling can be influenced by non-thermal electrons. Relaxation processes involving non-thermal electrons competing with the thermalized electron system have led to inconsistencies in the understanding of how electrons scatter and relax with the less energetic lattice. Recent theoretical and computational works have shown that the rate of energy relaxation with the metallic lattice will change depending on the thermalization state of the electrons. Even though 20 years of experimental works have focused on understanding and isolating these electronic relaxation mechanisms with short pulsed irradiation, discrepancies between these existing works have not clearly answered the fundamental question of the competing effects between non-thermal and thermal electrons losing energy to the lattice. In this work, we demonstrate the ability to measure the electron relaxation for varying degrees of both electron-electron and electron-phonon thermalization. This series of measurements of electronic relaxation over a predicted effective electron temperature range up to ∼3500 K and minimum lattice temperatures of 77 K validate recent computational and theoretical works that theorize how a nonequilibrium distribution of electrons transfers energy to the lattice. Utilizing this wide temperature range during pump-probe measurements of electron-phonon relaxation, we explain discrepancies in the past two decades of literature of electronic relaxation rates. We experimentally demonstrate that the electron-phonon coupling factor in gold increases with increasing lattice temperature and laser fluences. Specifically, we show that at low laser fluences corresponding to small electron perturbations, energy relaxation between electrons and phonons is mainly governed by non-thermal electrons, while at higher laser fluences, non-thermal electron scattering with the lattice is less influential on the energy relaxation
Structural Properties and Phonon dispertion of NACl
Directory of Open Access Journals (Sweden)
R. Khoda-Bakhsh
2001-06-01
Full Text Available Although many phenomena in condensed matter Physics can be understood on the basis of a model, there are also considerable number of physical properties of solid which can not be explained except in the framework of lattice dynamics. We have calculated the phonon frequencies of Na Cl, using an approach which is a combination of frozen phonon and force constants methods in the framework of density functional pseudopotential theory. The dispersion relation curves, were calculated along symmetry direction Δ, Σ and Ù. We also calculated Grunesein parameters for all modes at X and L points in Brillion zone. The calcutions are made in the framework of density functional and pseudopotential theory, using super cell method, with the valence orbitals expanded in plane waves.
Scattering of thermal phonons by extended defects in dielectric crystals
Energy Technology Data Exchange (ETDEWEB)
Roth, E. P.
1975-01-01
The scattering of thermal phonons by extended defects in dielectric crystals has been observed through measurements of thermal conductivity and ballistic heat pulse propagation. The thermal conductivities of LiF and NaCl conatining 500 low-angle grain boundaries per cm were measured in the range 0.08-5 K. The measurements gave little or no evidence for phonon scattering from the grain boundaries. Measurements of phonon scattering at a 10 deg. grain boundary in silicon using direct generation and detection of ballistically propagating heat pulses were made over an effective phonon temperature range of 2 to 20 K. The grain boundary reflection coefficient was determined to be < 2%. The thermal conductivities of LiF crystals containing 5 x 10/sup 6/ - 3 x 10/sup 7/ dislocations per square cm were measured over the temperature range 0.1 to 10 K. The measurements of the sheared crystal indicated that the slow transverse phonon mode was strongly scattered by a dynamic phonon-dislocation interaction at T approximately < 2 K, while the remaining modes were scattered primarily by the boundaries. The measurements of the bent crystals indicated that, for T approximately < 2 K, the slow transverse and possibly the longitudinal phonons were strongly scattered by a dynamic phonon-dislocation interaction. For T approximately > 2 k, some fraction of the phonons (at least the slow transverse mode) were still strongly scattered, even after long exposure to ..gamma.. irradiation, while the remaining phonons were scattered primarily by the boundaries.
Indian Academy of Sciences (India)
L Pintschovius; F Weber; W Reichardt; A Kreyssig; R Heid; D Reznik; O Stockert; K Hradil
2008-10-01
Phonons in a metal interact with conduction electrons which give rise to a finite linewidth. In the normal state, this leads to a Lorentzian shape of the phonon line. Density functional theory is able to predict the phonon linewidths as a function of wave vector for each branch of the phonon dispersion. An experimental verification of such predictions is feasible only for compounds with very strong electron–phonon coupling. YN2B2C was chosen as a test example because it is a conventional superconductor with a fairly high c (15.2 K). Inelastic neutron scattering experiments did largely confirm the theoretical predictions. Moreover, they revealed a strong temperature dependence of the linewidths of some phonons with particularly strong electron–phonon coupling which can as yet only qualitatively be accounted for by theory. For such phonons, marked changes of the phonon frequencies and linewidths were observed from room temperature down to 15 K. Further changes were observed on entering into the superconducting state. These changes can, however, not be described simply by a change of the phonon linewidth.
Theory of coherent phonons in carbon nanotubes and graphene nanoribbons
Sanders, G. D.; Nugraha, A. R. T.; Sato, K.; Kim, J.-H.; Kono, J.; Saito, R.; Stanton, C. J.
2013-04-01
We survey our recent theoretical studies on the generation and detection of coherent radial breathing mode (RBM) phonons in single-walled carbon nanotubes and coherent radial breathing like mode (RBLM) phonons in graphene nanoribbons. We present a microscopic theory for the electronic states, phonon modes, optical matrix elements and electron-phonon interaction matrix elements that allows us to calculate the coherent phonon spectrum. An extended tight-binding (ETB) model has been used for the electronic structure and a valence force field (VFF) model has been used for the phonon modes. The coherent phonon amplitudes satisfy a driven oscillator equation with the driving term depending on the photoexcited carrier density. We discuss the dependence of the coherent phonon spectrum on the nanotube chirality and type, and also on the graphene nanoribbon mod number and class (armchair versus zigzag). We compare these results with a simpler effective mass theory where reasonable agreement with the main features of the coherent phonon spectrum is found. In particular, the effective mass theory helps us to understand the initial phase of the coherent phonon oscillations for a given nanotube chirality and type. We compare these results to two different experiments for nanotubes: (i) micelle suspended tubes and (ii) aligned nanotube films. In the case of graphene nanoribbons, there are no experimental observations to date. We also discuss, based on the evaluation of the electron-phonon interaction matrix elements, the initial phase of the coherent phonon amplitude and its dependence on the chirality and type. Finally, we discuss previously unpublished results for coherent phonon amplitudes in zigzag nanoribbons obtained using an effective mass theory.
Electron-phonon coupling and the soft phonon mode in TiSe{<_2}.
Energy Technology Data Exchange (ETDEWEB)
Weber, F.; Rosenkranz, S.; Castellan, J.-P.; Osborn, R.; Karapetrov, G.; Hott, R.; Heid, R.; Bohnen, K.-P.; Alatas, A. (Materials Science Division); ( XSD); (Institut fur Festkorperphysik)
2011-01-01
We report high-resolution inelastic x-ray measurements of the soft phonon mode in the charge-density-wave compound TiSe{sub 2}. We observe a complete softening of a transverse optic phonon at the L point, i.e., q = (0.5,0,0.5), at T {approx} T{sub CDW}. Detailed ab initio calculations for the electronic and lattice dynamical properties of TiSe{sub 2} are in quantitative agreement with experimental frequencies for the soft phonon mode. The observed broad range of renormalized phonon frequencies, (0.3,0,0.5) {<=} q {<=} (0.5,0,0.5), is directly related to a broad peak in the electronic susceptibility stabilizing the charge-density-wave ordered state. Our analysis demonstrates that a conventional electron-phonon coupling mechanism can explain a structural instability and the charge-density-wave order in TiSe{sub 2} although other mechanisms might further boost the transition temperature.
Quantum Coherent Electron-Phonon Nanolaboratories
2006-05-31
published as “Single-crystal aluminum nitride nanomechanical resonators”, A.N. Cleland, M. Pophristic and I. Ferguson , Appl. Phys. Lett. 79, 2070 (2001...nanostructured phononic crystals”, Phys. Rev. B 64, 172301 (2001) A.N. Cleland, M. Pophristic and I. Ferguson , “Single-crystal aluminum nitride...Phys. Lett. 79, 1202 ~2001!. 6 M. J. Kelly, R. J. Brown, C. G. Smith, D. A. Wharam, M. Pepper , H. Ahmed, D. G. Hasko, D. C. Peacock, J. E. F. Frost, and
Quantum mode phonon forces between chainmolecules
DEFF Research Database (Denmark)
Bohr, Jakob
2001-01-01
A phenomenological description of the contributions of phonons to molecular force is developed. It uses an approximation to consider macromolecules as solid continua. The molecular modes of a molecule can then be characterized by a Debye-like description of the partition function. The resulting b....... For the later case, a significant change in zero-point energy is found. This may be the underlying cause for cold denaturation of proteins. (C) 2001 John Wiley & Sons, Inc....
Novel information theory techniques for phonon spectroscopy
Energy Technology Data Exchange (ETDEWEB)
Hague, J P [Department of Physics, Loughborough University, Loughborough, LE11 3TU (United Kingdom)
2007-12-15
The maximum entropy method (MEM) and spectral reverse Monte Carlo (SRMC) techniques are applied to the determination of the phonon density of states (PDOS) from heat-capacity data. The approach presented here takes advantage of the standard integral transform relating the PDOS with the specific heat at constant volume. MEM and SRMC are highly successful numerical approaches for inverting integral transforms. The formalism and algorithms necessary to carry out the inversion of specific heat curves are introduced, and where possible, I have concentrated on algorithms and experimental details for practical usage. Simulated data are used to demonstrate the accuracy of the approach. The main strength of the techniques presented here is that the resulting spectra are always physical: Computed PDOS is always positive and properly applied information theory techniques only show statistically significant detail. The treatment set out here provides a simple, cost-effective and reliable method to determine phonon properties of new materials. In particular, the new technique is expected to be very useful for establishing where interesting phonon modes and properties can be found, before spending time at large scale facilities.
Swinteck, Nichlas Z.
This dissertation contains research directed at investigating the behavior and properties of a class of composite materials known as phononic crystals. Two categories of phononic crystals are explicitly investigated: (I) elastic phononic crystals and (II) nano-scale phononic crystals. For elastic phononic crystals, attention is directed at two-dimensional structures. Two specific structures are evaluated (1) a two-dimensional configuration consisting of a square array of cylindrical Polyvinylchloride inclusions in air and (2) a two-dimensional configuration consisting of a square array of steel cylindrical inclusions in epoxy. For the first configuration, a theoretical model is developed to ascertain the necessary band structure and equi-frequency contour features for the realization of phase control between propagating acoustic waves. In contrasting this phononic crystal with a reference system, it is shown that phononic crystals with equifrequency contours showing non-collinear wave and group velocity vectors are ideal systems for controlling the phase between propagating acoustic waves. For the second configuration, it is demonstrated that multiple functions can be realized of a solid/solid phononic crystal. The epoxy/steel phononic crystal is shown to behave as (1) an acoustic wave collimator, (2) a defect-less wave guide, (3) a directional source for elastic waves, (4) an acoustic beam splitter, (5) a phase-control device and (6) a k-space multiplexer. To transition between macro-scale systems (elastic phononic crystals) and nano-scale systems (nano-phononic crystals), a toy model of a one-dimensional chain of masses connected with non-linear, anharmonic springs is utilized. The implementation of this model introduces critical ideas unique to nano-scale systems, particularly the concept of phonon mode lifetime. The nano-scale phononic crystal of interest is a graphene sheet with periodically spaced holes in a triangular array. It is found through equilibrium
High-Efficiency and High-Power Mid-Wave Infrared Cascade Lasers
2012-10-01
Black squares are lifetimes calculated by IFR scattering only. Red circles are lifetimes calculated by LO phonon scattering only. Blue triangles are...lifetimes taking into account of both IFR and LO phonon scattering. Different color shaded area represent different lasing wavelength regions. 55 vi...Approved for public release; distribution unlimited. 3.3 Calculated upper laser level lifetimes when both LO-phonon and IFR scattering are taken
Directory of Open Access Journals (Sweden)
X. Ding
2015-05-01
Full Text Available Thermal conductivity of ferroelastic device materials can be reversibly controlled by strain. The nucleation and growth of twin boundaries reduces thermal conductivity if the heat flow is perpendicular to the twin wall. The twin walls act as phonon barriers whereby the thermal conductivity decreases linearly with the number of such phonon barriers. Ferroelastic materials also show elasto-caloric properties with a high frequency dynamics. The upper frequency limit is determined by heat generation on a time scale, which is some 5 orders of magnitude below the typical bulk phonon times. Some of these nano-structural processes are irreversible under stress release (but remain reversible under temperature cycling, in particular the annihilation of needle domains that are a key indicator for ferroelastic behaviour in multiferroic materials.
Coupled bloch-phonon oscillations in semiconductor superlattices
Dekorsy; Bartels; Kurz; Kohler; Hey; Ploog
2000-07-31
We investigate coherent Bloch oscillations in GaAs/AlxGa1-xAs superlattices with electronic miniband widths larger than the optical phonon energy. In these superlattices the Bloch frequency can be tuned into resonance with the optical phonon. Close to resonance a direct coupling of Bloch oscillations to LO phonons is observed which gives rise to the coherent excitation of LO phonons. The density necessary for driving coherent LO phonons via Bloch oscillations is about 2 orders of magnitude smaller than the density necessary to drive coherent LO phonons in bulk GaAs. The experimental observations are confirmed by the theoretical description of this phenomenon [A.W. Ghosh et al., Phys. Rev. Lett. 85, 1084 (2000)].
Reduction of thermal conductivity by nanoscale 3D phononic crystal.
Yang, Lina; Yang, Nuo; Li, Baowen
2013-01-01
We studied how the period length and the mass ratio affect the thermal conductivity of isotopic nanoscale three-dimensional (3D) phononic crystal of Si. Simulation results by equilibrium molecular dynamics show isotopic nanoscale 3D phononic crystals can significantly reduce the thermal conductivity of bulk Si at high temperature (1000 K), which leads to a larger ZT than unity. The thermal conductivity decreases as the period length and mass ratio increases. The phonon dispersion curves show an obvious decrease of group velocities in 3D phononic crystals. The phonon's localization and band gap is also clearly observed in spectra of normalized inverse participation ratio in nanoscale 3D phononic crystal.
NATO Advanced Study Institute on Nonequilibrium Phonon Dynamics
1985-01-01
Phonons are always present in the solid state even at an absolute temperature of 0 K where zero point vibrations still abound. Moreover, phonons interact with all other excitations of the solid state and, thereby, influence most of its properties. Historically experimental information on phonon transport came from measurements of thermal conductivity. Over the past two decades much more, and much more detailed, information on phonon transport and on many of the inherent phonon interaction processes have come to light from experiments which use nonequilibrium phonons to study their dynamics. The resultant research field has most recently blossomed with the development of ever more sophisticated experimental and theoretical methods which can be applied to it. In fact, the field is moving so rapidly that new members of the research community have difficulties in keeping up to date. This NATO Advanced Study Institute (ASI) was organized with the objective of overcoming the information barrier between those expert...
Phonon Scattering Dynamics of Thermophoretic Motion in Carbon Nanotube Oscillators.
Prasad, Matukumilli V D; Bhattacharya, Baidurya
2016-04-13
Using phonon wave packet molecular dynamics simulations, we find that anomalous longitudinal acoustic (LA) mode phonon scattering in low to moderate energy ranges is responsible for initiating thermophoretic motion in carbon nanotube oscillators. The repeated scattering of a single mode LA phonon wave packet near the ends of the inner nanotube provides a net unbalanced force that, if large enough, initiates thermophoresis. By applying a coherent phonon pulse on the outer tube, which generalizes the single mode phonon wave packet, we are able to achieve thermophoresis in a carbon nanotube oscillator. We also find the nature of the unbalanced force on end-atoms to be qualitatively similar to that under an imposed thermal gradient. The thermodiffusion coefficient obtained for a range of thermal gradients and core lengths suggest that LA phonon scattering is the dominant mechanism for thermophoresis in longer cores, whereas for shorter cores, it is the highly diffusive mechanism that provides the effective force.
Raman spectra of semiconductor nanoparticles: Disorder-activated phonons
Ingale, Alka; Rustagi, K. C.
1998-09-01
We present Raman spectra of four semiconductor doped glasses and a single crystal of CdS0.55Se0.45 in the range 30-800 cm-1 in the backscattering geometry. This includes the first-order Raman scattering from the disorder-activated zone-edge phonons and the LO phonons. TO phonon modes are not observed, as in bulk CdS, for the excitation well above the lowest gap. We show that the asymmetric line profile of the LO phonon structure can be understood as a composite of two phonon modes: the zone center and the zone edge phonons. Disorder-activated modes in the (30-130)-cm-1 range and the higher-order Raman spectra are also observed and found to be consistent with this assignment.
Interaction of excitons with optical phonons in layer crystals
Nitsovich, Bohdan M.; Zenkova, C. Y.; Kramar, N. K.
2002-02-01
The investigation is concerned with layer crystals of the GaSe, InSe, GaTe, MoS2-type and other inorganic semiconductors, whose phonon spectrum has a great number of peculiarities, among them the availability of low-energy optical phonons. In this case the dispersion of these phonons can be essential and vary in character. The mass operator of the exciton-phonon system and the light absorption coefficient for different dispersion laws of optical phonons have been calculated. The influence of the sign of the phonon 'effective mass' on the exciton absorption band of layer crystals, which causes the opposite in sign dynamics of the absorption maximum shift, and the change of the absorption curve asymmetry have been determined.
Weak phonon scattering effect of twin boundaries on thermal transmission.
Dong, Huicong; Xiao, Jianwei; Melnik, Roderick; Wen, Bin
2016-01-29
To study the effect of twin boundaries on thermal transmission, thermal conductivities of twinned diamond with different twin thicknesses have been studied by NEMD simulation. Results indicate that twin boundaries show a weak phonon scattering effect on thermal transmission, which is only caused by the additional twin boundaries' thermal resistance. Moreover, according to phonon kinetic theory, this weak phonon scattering effect of twin boundaries is mainly caused by a slightly reduced average group velocity.
Weak phonon scattering effect of twin boundaries on thermal transmission
Huicong Dong; Jianwei Xiao; Roderick Melnik; Bin Wen
2016-01-01
To study the effect of twin boundaries on thermal transmission, thermal conductivities of twinned diamond with different twin thicknesses have been studied by NEMD simulation. Results indicate that twin boundaries show a weak phonon scattering effect on thermal transmission, which is only caused by the additional twin boundaries’ thermal resistance. Moreover, according to phonon kinetic theory, this weak phonon scattering effect of twin boundaries is mainly caused by a slightly reduced averag...
Isotopic effects on the phonon modes in boron carbide.
Werheit, H; Kuhlmann, U; Rotter, H W; Shalamberidze, S O
2010-10-01
The effect of isotopes ((10)B-(11)B; (12)C-(13)C) on the infrared- and Raman-active phonons of boron carbide has been investigated. For B isotopes, the contributions of the virtual crystal approximation, polarization vector and isotopical disorder are separated. Boron and carbon isotope effects are largely opposite to one another and indicate the share of the particular atoms in the atomic assemblies vibrating in specific phonon modes. Some infrared-active phonons behave as expected for monatomic boron crystals.
Interface phonon effect on optical spectra of quantum nanostructures
Energy Technology Data Exchange (ETDEWEB)
Maslov, Alexander Yu., E-mail: maslov.ton@mail.ioffe.r [Ioffe Physical Technical Institute, Polytechnicheskaya st., 26, 194021 Saint Petersburg (Russian Federation); Proshina, Olga V.; Rusina, Anastasia N. [Ioffe Physical Technical Institute, Polytechnicheskaya st., 26, 194021 Saint Petersburg (Russian Federation)
2009-12-15
This paper deals with theory of large radius polaron effect in quantum wells, wires and dots. The interaction of charge particles and excitons with both bulk and interface optical phonons is taken into consideration. The analytical expression for polaron binding energy is obtained for different types of nanostructures. It is shown that the contribution of interface phonons to the polaron binding energy may exceed the bulk phonon part. The manifestation of polaron effects in optical spectra of quantum nanostructures is discussed.
DEFF Research Database (Denmark)
Angelsky, O. V.; Bekshaev, A. Ya.; Maksimyak, P. P.;
2014-01-01
-diffraction of the incident light, here being strongly sensitive to the medium position with respect to the focus. This technique, based on the complex spatial structure of both the incident and the diffracted fields, can be employed for the detection and measurement of weak non-linearities.......Water suspension of light-absorbing nano-sized particles is an example of a medium in which non-linear effects are present at moderate light intensities favorable for optical treatment of organic and biological objects. We study experimentally the phenomena emerging in a thin layer of such a medium...... under the action of inhomogeneous light field formed due to the Pearcey diffraction pattern near a microlens focus. In this high-gradient field, the light energy absorbed by the particles induces inhomogeneous distribution of the medium refraction index, which results in observable self...
Phonon dispersion and lifetimes in MgB2.
Shukla, Abhay; Calandra, Matteo; D'Astuto, Matteo; Lazzeri, Michele; Mauri, Francesco; Bellin, Christophe; Krisch, Michael; Karpinski, J; Kazakov, S M; Jun, J; Daghero, D; Parlinski, K
2003-03-01
We measure phonon dispersion and linewidth in a single crystal of MgB2 along the Gamma-A, Gamma-M, and A-L directions using inelastic x-ray scattering. We use density functional theory to compute the effect of both electron-phonon coupling and anharmonicity on the linewidth, obtaining excellent agreement with experiment. Anomalous broadening of the E(2g) phonon mode is found all along Gamma-A. The dominant contribution to the linewidth is always the electron-phonon coupling.
Engineering interactions between superconducting qubits and phononic nanostructures
Arrangoiz-Arriola, Patricio; Safavi-Naeini, Amir H.
2016-12-01
Nanomechanical systems can support highly coherent microwave-frequency excitations at cryogenic temperatures. However, generating sufficient coupling between these devices and superconducting quantum circuits is challenging due to the vastly different length scales of acoustic and electromagnetic excitations. Here we demonstrate a general method for calculating piezoelectric interactions between quantum circuits and arbitrary phononic nanostructures. We illustrate our technique by studying the coupling between a transmon qubit and bulk acoustic-wave, Lamb-wave, and phononic crystal resonators, and show that very large coupling rates are possible in all three cases. Our results suggest a route to phononic circuits and systems that are nonlinear at the single-phonon level.
Phononic glass: a robust acoustic-absorption material.
Jiang, Heng; Wang, Yuren
2012-08-01
In order to achieve strong wide band acoustic absorption under high hydrostatic pressure, an interpenetrating network structure is introduced into the locally resonant phononic crystal to fabricate a type of phononic composite material called "phononic glass." Underwater acoustic absorption coefficient measurements show that the material owns high underwater sound absorption coefficients over 0.9 in 12-30 kHz. Moreover, the quasi-static compressive behavior shows that the phononic glass has a compressive strength over 5 MPa which is crucial for underwater applications.
Bloch oscillations in the presence of plasmons and phonons
Ghosh; Jonsson; Wilkins
2000-07-31
The coupling between Bloch oscillating electrons and longitudinal optical phonons in a superlattice leads to resonant phonon excitation but no gap in the Bloch-phonon spectrum. In addition, we predict a sharp transition from plasma to Bloch oscillations at nu(B) = 2nu(P). From a microscopic description with phenomenological dampings, we numerically map out the behavior of coupled Bloch-plasmon-phonon modes for a wide range of parameters, and mimic experimental conditions. Our results are in good agreement with recent experiments by Dekorsy et al. [Phys. Rev. Lett. 85, 1080 (2000)].
Multi-phonon dynamics of the ultra-fast photoinduced transition of (EDO-TTF)2SbF6
Lorenc, Maciej; Moisan, Nicolas; Servol, Marina; Cailleau, Hervé; Koshihara, Shin-ya; Maesato, Mitsuhiko; Shao, Xiangfeng; Nakano, Yoshiaki; Yamochi, Hideki; Saito, Gunzi; Collet, Eric
2009-02-01
We report here the first observation of the photoinduced insulating-to-metal phase transition in the (EDO-TTF)2SbF6 salt, which occurs on the picosecond time-scale. The time-resolved optical experiments performed with 80 fs time-resolution demonstrate that the dynamical process involves several low-frequency phonons, as the crystalline structure is destabilized upon laser excitation.
Watanabe, Yohei; Hino, Ken-Ichi; Hase, Muneaki; Maeshima, Nobuya
The coherent phonon (CP) generation is one of the representative phenomena induced by ultrashort pulsed laser. In particular, in the initial stage of the CP generation in lightly n-doped Si, the vestige of Fano resonance (FR) manifested in a flash was observed in time-resolved spectroscopy experiments, in which it was speculated that this phenomenon results from the birth of transient polaronic quasiparticles composed of electrons and phonons strongly interacting each other. This study is aimed at constructing a fully-quantum-mechanical model for the CP generation and tracking the origin of the transient FR. We calculate two physical quantities in both of polar and non-polar semiconductors such as GaAs and undoped Si. One is a retarded longitudinal susceptibility which allows one to calculate a transient induced photoemission spectrum. The other is the Fourier-transform of LO-phonon displacement into frequency domain. We have succeeded in showing that the transient FR is exclusively caused in Si in harmony with the experiments, though, not observed in GaAs.
Dynamical control of electron-phonon interactions with high-frequency light
Dutreix, C.; Katsnelson, M. I.
2017-01-01
This work addresses the one-dimensional problem of Bloch electrons when they are rapidly driven by a homogeneous time-periodic light and linearly coupled to vibrational modes. Starting from a generic time-periodic electron-phonon Hamiltonian, we derive a time-independent effective Hamiltonian that describes the stroboscopic dynamics up to the third order in the high-frequency limit. This yields nonequilibrium corrections to the electron-phonon coupling that are controllable dynamically via the driving strength. This shows in particular that local Holstein interactions in equilibrium are corrected by antisymmetric Peierls interactions out of equilibrium, as well as by phonon-assisted hopping processes that make the dynamical Wannier-Stark localization of Bloch electrons impossible. Subsequently, we revisit the Holstein polaron problem out of equilibrium in terms of effective Green's functions, and specify explicitly how the binding energy and effective mass of the polaron can be controlled dynamically. These tunable properties are reported within the weak- and strong-coupling regimes since both can be visited within the same material when varying the driving strength. This work provides some insight into controllable microscopic mechanisms that may be involved during the multicycle laser irradiations of organic molecular crystals in ultrafast pump-probe experiments, although it should also be suitable for realizations in shaken optical lattices of ultracold atoms.
Energy Technology Data Exchange (ETDEWEB)
Souvatzis, P; Rudin, S P [Theoretical Division, Los Alamos National Laboratory, Los Alamos, NM 87545 (United States); Bjoerkman, T; Eriksson, O [Department of Physics, Uppsala University, Box 530, SE-75121, Uppsala (Sweden); Andersson, P [FOI, Swedish Defence Research Agency, SE-164 90 Stockholm (Sweden); Katsnelson, M I [Institute for Molecules and Materials, Radboud University Nijmegen, NL-6525 ED, Nijmegen (Netherlands)], E-mail: petros.souvatzis@gmail.com
2009-04-29
A recently developed self-consistent ab initio lattice dynamical method has been applied to the high temperature body centered cubic (bcc) phase of La and Th, which are dynamically unstable at low temperatures. The bcc phase of these metals is found to be stabilized by phonon-phonon interactions. The calculated high temperature phonon frequencies for La are found to be in good agreement with the corresponding experimental data.
Rabi oscillations in a quantum dot-cavity system coupled to a nonzero temperature phonon bath
Energy Technology Data Exchange (ETDEWEB)
Larson, Jonas [ICFO-Institut de Ciencies Fotoniques, E-08860 Castelldefels, Barcelona (Spain); Moya-Cessa, Hector [INAOE, Coordinacion de Optica, Apdo. Postal 51 y 216, 72000 Puebla, Pue (Mexico)], E-mail: jolarson@kth.se
2008-06-15
We study a quantum dot strongly coupled to a single high-finesse optical microcavity mode. We use a rotating wave approximation (RWA) method, commonly used in ion-laser interactions, together with the Lamb-Dicke approximation to obtain an analytic solution of this problem. The decay of Rabi oscillations because of the electron-phonon coupling is studied at arbitrary temperature and analytical expressions for the collapse and revival times are presented. Analyses without the RWA are presented as means of investigating the energy spectrum.
Resonant behaviour of GaAs LO phonons in a GaAs-AlAs superlattice
Zhang, Shulin; T, A. Gant; M, Delaney; M, V. Klein; J, Klem; H, Morkoc
1988-03-01
Resonant Raman scattering from GaAs LO phonons in a 59Å GaAs/20Å AlAs superlattice was studied. The relevant intersubband energies were determined. The results suggest that all of the exciton transitions from the hole subbands HH1, LH1, HH2, HH3, LH2 and HH4 to the electron subbands CB1 and CB2 in the energy region covered by our incident dye laser were observed and a justificative analysis may involve effects due to valence band mixing and to 3D electronic miniband structure.
Coherent phonon spectroscopy of non-fully symmetric modes using resonant terahertz excitation
Energy Technology Data Exchange (ETDEWEB)
Huber, T., E-mail: tihuber@phys.ethz.ch; Huber, L.; Johnson, S. L. [Institute for Quantum Electronics, Physics Department, ETH Zurich, CH-8093 Zurich (Switzerland); Ranke, M. [The Hamburg Centre for Ultrafast Imaging, Luruper Chaussee 149, D-22761 Hamburg (Germany); Ferrer, A. [Institute for Quantum Electronics, Physics Department, ETH Zurich, CH-8093 Zurich (Switzerland); Swiss Light Source, Paul Scherrer Institut, CH-5232 Villigen PSI (Switzerland)
2015-08-31
We use intense terahertz (THz) frequency electromagnetic pulses generated via optical rectification in an organic crystal to drive vibrational lattice modes in single crystal Tellurium. The coherent modes are detected by measuring the polarization changes of femtosecond laser pulses reflecting from the sample surface, resulting in a phase-resolved detection of the coherent lattice motion. We compare the data to a model of Lorentz oscillators driven by the near-single-cycle broadband THz pulse. The demonstrated technique of optically probed coherent phonon spectroscopy with THz frequency excitation could prove to be a viable alternative to other time-resolved spectroscopic methods like standard THz time domain spectroscopy.
Hypersonic modulation of light in three-dimensional photonic and phononic band-gap materials.
Akimov, A V; Tanaka, Y; Pevtsov, A B; Kaplan, S F; Golubev, V G; Tamura, S; Yakovlev, D R; Bayer, M
2008-07-18
The elastic coupling between the a-SiO2 spheres composing opal films brings forth three-dimensional periodic structures which besides a photonic stop band are predicted to also exhibit complete phononic band gaps. The influence of elastic crystal vibrations on the photonic band structure has been studied by injection of coherent hypersonic wave packets generated in a metal transducer by subpicosecond laser pulses. These studies show that light with energies close to the photonic band gap can be efficiently modulated by hypersonic waves.
Conductivity of strongly pumped superconductors. An electron-phonon system far from equilibrium
Energy Technology Data Exchange (ETDEWEB)
Krull, Holger
2015-01-29
The study of nonequilibrium physics is of great interest, because one can capture novel phenomena and properties which are hidden at equilibrium, e.g., one can study relaxation processes. A common way to study the nonequilibrium dynamics of a sample is a pump-probe experiment. In a pump probe experiment an intense laser pulse, the so called pump pulse, excites the sample and takes it out of equilibrium. After a certain delay time a second pulse, the probe pulse, measures the actual state of the sample. In this thesis, we theoretically study the pump-probe response of superconductors. On the one hand we are interest in the effect of a pump pulse and on the other hand we want to provide the pump-probe response, such that experimental measurement can be easily interpreted. In order to do this, we use the density matrix formalism to compute the pump-probe response of the system. In the density matrix formalism equations of motion are set up for expectation values of interest. In order to study the dynamics induced by a pump pulse, we compute the temporal evolution of the quasiparticle densities and the mean phonon amplitude. We find that the induced dynamics of the system depends on characteristics of the pump pulse. For short pulses, the system is pushed into the nonadiabatic regime. In this regime, the order parameter is lowered during the pump pulse and shows a 1/(√(t))-decaying oscillation afterwards. In addition, coherent phonons are generated, which is resonantly enhanced if the frequency of the order parameter oscillation is equal to the phonon frequency. For long pulses, the system is pushed into the adiabatic regime. In this regime, the order parameter is lowered during the pulse and remains almost constant afterwards. Further, there is almost no generation of coherent phonons. For the pump-probe response we compute the conductivity induced by the probe pulse. The conductivity is a typical observable in real pump-probe experiments. Hence, it is possible to
Phonon excitations and magnetoelectric coupling in multiferroic RMn2O5
Golrokh Bahoosh, Safa; Wesselinowa, Julia M.; Trimper, Steffen
2013-05-01
Multiferroic rare-earth manganites are theoretically studied by focusing on the coupling to the lattice degrees of freedom. We demonstrate analytically that the phonon excitations in the multiferroic phase are strongly affected by the magnetoelectric coupling, the spin-phonon interaction and the anharmonic phonon-phonon interaction. Based on a microscopic model, the temperature dependence of the phonon dispersion relation is analyzed. It offers an anomaly at both the ferroelectric and the magnetic transition indicating the mutual coupling between multiferroic orders and lattice distortions. Depending on the sign of the spin-phonon coupling the phonon modes become softer or harder in accordance with experimental observations. We show that the phonon spectrum can be also controlled by an external magnetic field. The phonon energy is enhanced by increasing that field. The applied Green's function technique allows the calculation of the macroscopic magnetization depending on both the phonon-phonon and the spin-phonon couplings.
Coherent phonon optics in a chip with an electrically controlled active device.
Poyser, Caroline L; Akimov, Andrey V; Campion, Richard P; Kent, Anthony J
2015-02-05
Phonon optics concerns operations with high-frequency acoustic waves in solid media in a similar way to how traditional optics operates with the light beams (i.e. photons). Phonon optics experiments with coherent terahertz and sub-terahertz phonons promise a revolution in various technical applications related to high-frequency acoustics, imaging, and heat transport. Previously, phonon optics used passive methods for manipulations with propagating phonon beams that did not enable their external control. Here we fabricate a phononic chip, which includes a generator of coherent monochromatic phonons with frequency 378 GHz, a sensitive coherent phonon detector, and an active layer: a doped semiconductor superlattice, with electrical contacts, inserted into the phonon propagation path. In the experiments, we demonstrate the modulation of the coherent phonon flux by an external electrical bias applied to the active layer. Phonon optics using external control broadens the spectrum of prospective applications of phononics on the nanometer scale.
Phonons in Quantum-Dot Quantum Well
Institute of Scientific and Technical Information of China (English)
QINGuo-Yi
2004-01-01
Phonon modes of A1As/GaAs/A1As and GaAs/A1As/metal Pb quantum-dot quantum wells (QDQW's) with the whole scale up to 90 AО are calculated by using valence force field model (VFFM) based on group theory.Their optical frequency spectra are divided into two nonoverlapping bands, the AlAs-like band and the GaAs-like band,originated from and having frequency interval inside the bulk AlAs optical band and bulk GaAs optical band, respectively.The GaAs-LO (Г)-like modes of QDQW's that have maximum bulk GaAs-LO (Г) parentages in all modes covering thewhole frequency region and all symmetries have always A1 symmetry. Its frequency is controllable by adjusting thestructure parameters. In A1As/GaAs/A1As, it may be controlled to meet any designed frequency in GaAs-like band.The results on GaAs/A1As/metal Pb QDQW's show the same effect of reducing in interface optical phonons by using the metal/semiconductor interface revealed ever by macroscopic model The frequency spectra in both GaAs-like andAlAs-like optical phonon bands are independent of the thickness of Pb shell as long as the thickness of Pb shell is no less than 5 AО Defects at metal/A1As interface have significant influence to AlAs-like optical modes but have only minor influence to GaAs-like optical modes. All these results are important for the studying of the e-ph interaction in QD structures.
Phonons in Quantum-Dot Quantum Well
Institute of Scientific and Technical Information of China (English)
QIN Guo-Yi
2004-01-01
Phonon modes of AlAs/GaAs/AlAs and GaAs/AlAs/metal Pb quantum-dot quantum wells (QDQW's)with the whole scale up to 90 A are calculated by using valence force field model (VFFM) based on group theory.Their optical frequency spectra are divided into two nonoverlapping bands, the AMs-like band and the GaAs-like band,originated from and having frequency interval inside the bulk AlAs optical band and bulk GaAs optical band, respectively.The GaAs-LO (F)-like modes of QDQW's that have maximum bulk GaAs-LO (F) parentages in all modes covering the whole frequency region and all symmetries have always A1 symmetry. Its frequency is controllable by adjusting the structure parameters. In AlAs/GaAs/AlAs, it may be controlled to meet any designed frequency in GaAs-like band.The results on GaAs/AMs/metal Pb QDQW's show the same effect of reducing in interface optical phonons by using the metal/semiconductor interface revealed ever by macroscopic model. The frequency spectra in both GaAs-like and AlAs-like optical phonon bands are independent of the thickness of Pb shell as long as the thickness of Pb shell is no less than 5 A. Defects at metal/AlAs interface have significant influence to AMs-like optical modes but have only minor influence to GaAs-like optical modes. All these results are important for the studying of the e-ph interaction in QD structures.
Optimizing phonon-cooled Nb hot-electron bolometers
Araújo, H. M.; Puplett, E. F.; White, G. J.
2000-12-01
A Nb hot-electron bolometer designed for operation as a sensor of millimeter waves and far-infrared radiation has been analyzed. This optically coupled detector has a very wide spectral bandwidth, a response speed of ˜1 ns determined by electron-phonon scattering, and an impedance of 50 Ω. The geometry employed here has traditionally been affected by stability problems manifesting as random voltage fluctuations, which have hindered the usefulness of these bolometers. This issue has been addressed by exploring the underlying physical causes and adapting the fabrication technique. Analytical results on substrate-induced bolometric effects are summarized and other factors concerning detector performance addressed, and the reality of an isothermal regime of operation is questioned. A noise equivalent power of 4 pW/Hz1/2 was measured at 100 μm, with a coupling efficiency close to unity that was achieved by reducing the optical reflection losses. Operation of a similar device is shown able to resolve the macropulses of FELIX, the Free-Electron Laser for Infrared eXperiments, into its 40 ns spaced micropulses.
Semi-Dirac points in phononic crystals
Zhang, Xiujuan
2014-01-01
A semi-Dirac cone refers to a peculiar type of dispersion relation that is linear along the symmetry line but quadratic in the perpendicular direction. It was originally discovered in electron systems, in which the associated quasi-particles are massless along one direction, like those in graphene, but effective-mass-like along the other. It was reported that a semi-Dirac point is associated with the topological phase transition between a semi-metallic phase and a band insulator. Very recently, the classical analogy of a semi-Dirac cone has been reported in an electromagnetic system. Here, we demonstrate that, by accidental degeneracy, two-dimensional phononic crystals consisting of square arrays of elliptical cylinders embedded in water are also able to produce the particular dispersion relation of a semi-Dirac cone in the center of the Brillouin zone. A perturbation method is used to evaluate the linear slope and to affirm that the dispersion relation is a semi-Dirac type. If the scatterers are made of rubber, in which the acoustic wave velocity is lower than that in water, the semi-Dirac dispersion can be characterized by an effective medium theory. The effective medium parameters link the semi-Dirac point to a topological transition in the iso-frequency surface of the phononic crystal, in which an open hyperbola is changed into a closed ellipse. This topological transition results in drastic change in wave manipulation. On the other hand, the theory also reveals that the phononic crystal is a double-zero-index material along the x-direction and photonic-band-edge material along the perpendicular direction (y-direction). If the scatterers are made of steel, in which the acoustic wave velocity is higher than that in water, the effective medium description fails, even though the semi-Dirac dispersion relation looks similar to that in the previous case. Therefore different wave transport behavior is expected. The semi-Dirac points in phononic crystals described in
Phonon scattering in graphene over substrate steps
Energy Technology Data Exchange (ETDEWEB)
Sevinçli, H., E-mail: haldunsevincli@iyte.edu.tr [Department of Materials Science and Engineering, Izmir Institute of Technology, Gülbahçe Kampüsü, 35430 Urla, Izmir (Turkey); Department of Micro- and Nano-technology (DTU Nanotech), Technical University of Denmark, DK-2800 Kongens Lyngby (Denmark); Brandbyge, M., E-mail: mads.brandbyge@nanotech.dtu.dk [Department of Micro- and Nano-technology (DTU Nanotech), Technical University of Denmark, DK-2800 Kongens Lyngby (Denmark); Center for Nanostructured Graphene(CNG), Department of Micro- and Nano-technology, Technical University of Denmark, DK-2800 Kongens Lyngby (Denmark)
2014-10-13
We calculate the effect on phonon transport of substrate-induced bends in graphene. We consider bending induced by an abrupt kink in the substrate, and provide results for different step-heights and substrate interaction strengths. We find that individual substrate steps reduce thermal conductance in the range between 5% and 47%. We also consider the transmission across linear kinks formed by adsorption of atomic hydrogen at the bends and find that individual kinks suppress thermal conduction substantially, especially at high temperatures. Our analysis show that substrate irregularities can be detrimental for thermal conduction even for small step heights.
Large scale phononic metamaterials for seismic isolation
Energy Technology Data Exchange (ETDEWEB)
Aravantinos-Zafiris, N. [Department of Sound and Musical Instruments Technology, Ionian Islands Technological Educational Institute, Stylianou Typaldou ave., Lixouri 28200 (Greece); Sigalas, M. M. [Department of Materials Science, University of Patras, Patras 26504 (Greece)
2015-08-14
In this work, we numerically examine structures that could be characterized as large scale phononic metamaterials. These novel structures could have band gaps in the frequency spectrum of seismic waves when their dimensions are chosen appropriately, thus raising the belief that they could be serious candidates for seismic isolation structures. Different and easy to fabricate structures were examined made from construction materials such as concrete and steel. The well-known finite difference time domain method is used in our calculations in order to calculate the band structures of the proposed metamaterials.
Spectroscopy of nonequilibrium electrons and phonons
Shank, CV
1992-01-01
The physics of nonequilibrium electrons and phonons in semiconductors is an important branch of fundamental physics that has many practical applications, especially in the development of ultrafast and ultrasmall semiconductor devices. This volume is devoted to different trends in the field which are presently at the forefront of research. Special attention is paid to the ultrafast relaxation processes in bulk semiconductors and two-dimensional semiconductor structures, and to their study by different spectroscopic methods, both pulsed and steady-state. The evolution of energy and space distrib
TOPICAL REVIEW: Interaction of coherent phonons with defects and elementary excitations
Hase, Muneaki; Kitajima, Masahiro
2010-02-01
We present an overview of the feasibility of using coherent phonon spectroscopy to study interaction dynamics of excited lattice vibrations with their environments. By exploiting the features of coherent phonons with a pump-probe technique, one can study lattice motions in a sub-picosecond time range. The dephasing properties tell us not only about interaction dynamics with carriers (electrons and holes) or thermal phonons but also about point defects in crystals. Modulations of the coherent phonon amplitude by more than two modes are closely related to phonon-carrier or phonon-phonon interferences. Related to this phenomenon, formation of coherent phonons at higher harmonics gives direct evidence for phonon-phonon couplings. A combined study of coherent phonons and ultrafast carrier response can be useful for understanding phonon-carrier interaction dynamics. For metals like zinc, nonequilibrium electrons may dominate the dynamics of both relaxation and generation of coherent phonons. The frequency chirp of coherent phonons can be a direct measure of how and when phonon-phonon and phonon-carrier couplings occur. Carbon nanotubes show some complicated behavior due to the existence of many modes with different symmetries, resulting in superposition or interference. To illustrate one of the most interesting applications, the selective excitation of specific phonon modes through the use of a pulse train technique is shown.
Phonon excitation and instabilities in biased graphene nanoconstrictions
DEFF Research Database (Denmark)
Gunst, Tue; Lu, Jing Tao; Hedegård, Per;
2013-01-01
We investigate how a high current density perturbs the phonons in a biased graphene nanoconstriction coupled to semi-infinite electrodes. The coupling to electrode phonons, electrode electrons under bias, Joule heating, and current-induced forces is evaluated using first principles density...
First-principles dynamics of electrons and phonons
Bernardi, Marco
2016-01-01
First-principles calculations combining density functional theory and many-body perturbation theory can provide microscopic insight into the dynamics of electrons and phonons in materials. We review this theoretical and computational framework, focusing on perturbative treatments of scattering, dynamics and transport of coupled electrons and phonons. We discuss application of these first-principles calculations to electronics, lighting, spectroscopy and renewable energy.
Remarkable reduction of thermal conductivity in phosphorene phononic crystal.
Xu, Wen; Zhang, Gang
2016-05-05
Phosphorene has received much attention due to its interesting physical and chemical properties, and its potential applications such as thermoelectricity. In thermoelectric applications, low thermal conductivity is essential for achieving a high figure of merit. In this work, we propose to reduce the thermal conductivity of phosphorene by adopting the phononic crystal structure, phosphorene nanomesh. With equilibrium molecular dynamics simulations, we find that the thermal conductivity is remarkably reduced in the phononic crystal. Our analysis shows that the reduction is due to the depressed phonon group velocities induced by Brillouin zone folding, and the reduced phonon lifetimes in the phononic crystal. Interestingly, it is found that the anisotropy ratio of thermal conductivity could be tuned by the 'non-square' pores in the phononic crystal, as the phonon group velocities in the direction with larger projection of pores is more severely suppressed, leading to greater reduction of thermal conductivity in this direction. Our work provides deep insight into thermal transport in phononic crystals and proposes a new strategy to reduce the thermal conductivity of monolayer phosphorene.
Suppression of phonon transport in molecular Christmas trees.
Lambert, Colin John; Famili, Marjan; Grace, Iain; Sadeghi, Hatef
2017-02-27
Minimising the phonon thermal conductance of self-assembled molecular films, whilst preserving their electrical properties, is highly desirable, both for thermal management at the nanoscale and for the design of high-efficiency thermoelectric materials. Here we highlight a new strategy for minimising the phonon thermal conductance of Christmas-tree-like molecules composed of a long trunk, along which phonons can propagate, attached to pendant molecular branches. We demonstrate that phonon transport along the trunk is suppressed by Fano resonances associated with internal vibrational modes of the branches and that thermal conductance is suppressed most-effectively in molecules with pendant branches of different lengths. As examples, we use density functional theory to demonstrate the reduction in phonon transport in tree-like molecules formed from alkane or acene trunks with various pendant branches.
Phononic Frequency Comb via Intrinsic Three-Wave Mixing
Ganesan, Adarsh; Do, Cuong; Seshia, Ashwin
2017-01-01
Optical frequency combs have resulted in significant advances in optical frequency metrology and found wide applications in precise physical measurements and molecular fingerprinting. A direct analogue of frequency combs in the phononic or acoustic domain has not been reported to date. In this Letter, we report the first clear experimental evidence for a phononic frequency comb. We show that the phononic frequency comb is generated through the intrinsic coupling of a driven phonon mode with an autoparametrically excited subharmonic mode. The experiments depict the comb generation process evidenced by a spectral response consisting of equally spaced discrete and phase coherent comb lines. Through systematic experiments at different drive frequencies and amplitudes, we portray the well-connected process of phononic frequency comb formation and define the attributes to control the features associated with comb formation in such a system. In addition to the demonstration of frequency comb, the interplay between the nonlinear resonances and the well-known Duffing phenomenon is also observed.
Finite element analysis of surface modes in phononic crystal waveguides
Guo, Yuning; Schubert, Martin; Dekorsy, Thomas
2016-03-01
The study of surface modes in phononic crystal waveguides in the hypersonic regime is a burgeoning field with a large number of possible applications. By using the finite element method, the band structure and the corresponding transmission spectrum of surface acoustic waves in phononic crystal waveguides generated by line defects in a silicon pillar-substrate system were calculated and investigated. The bandgaps are caused by the hybridization effect of band branches induced by local resonances and propagating modes in the substrate. By changing the sizes of selected pillars in the phononic crystal waveguides, the corresponding bands shift and localized modes emerge due to the local resonance effect induced by the pillars. This effect offers further possibilities for tailoring the propagation and filtering of elastic waves. The presented results have implications for the engineering of phonon dynamics in phononic nanostructures.
Heterobarrier for converting hot-phonon energy to electric potential
Shin, Seungha; Melnick, Corey; Kaviany, Massoud
2013-02-01
We show that hot phonons emitted in energy conversion or resistive processes can be converted to electric potential in heterobarrier structures. Using phonon and electron interaction kinetics and self-consistent ensemble Monte Carlo, we find the favorable conditions for unassisted absorption of hot phonons and design graded heterobarriers for their direct conversion into electric energy. Tandem barriers with nearly optical-phonon height allow for substantial potential gain without current loss. We find that 19% of hot phonons can be harvested with an optimized GaAs/AlxGa1-xAs barrier structure over a range of current and electron densities, thus enhancing the overall energy conversion efficiency and reducing waste heat.
Controlling elastic waves with small phononic crystals containing rigid inclusions
Peng, Pai
2014-05-01
We show that a two-dimensional elastic phononic crystal comprising rigid cylinders in a solid matrix possesses a large complete band gap below a cut-off frequency. A mechanical model reveals that the band gap is induced by negative effective mass density, which is affirmed by an effective medium theory based on field averaging. We demonstrate, by two examples, that such elastic phononic crystals can be utilized to design small devices to control low-frequency elastic waves. One example is a waveguide made of a two-layer anisotropic elastic phononic crystal, which can guide and bend elastic waves with wavelengths much larger than the size of the waveguide. The other example is the enhanced elastic transmission of a single-layer elastic phononic crystal loaded with solid inclusions. The effective mass density and reciprocal of the modulus of the single-layer elastic phononic crystal are simultaneously near zero. © CopyrightEPLA, 2014.
Quantum noise theory for phonon transport through nanostructures
Wan, Li; Huang, Yunmi; Huang, Changcheng
2017-04-01
We have developed a quantum noise approach to study the phonon transport through nanostructures. The nanostructures acting as phonon channels are attached to two phonon reservoirs. And the temperature drop between the two reservoirs drives the phonon transport through the channels. We have derived a quantum Langevin equation(QLE) to describe the phonon transport with the quantum noise originated from the thermal fluctuation of the reservoirs. Within the Markov approximation, the QLE is used to get the thermal conductivity κ of the nanostructures and the finite size effect of the κ then is studied. In this study, the advantage of the quantum noise approach lays on the fact that no any local temperature needs to be defined for the nanostructures in its non-equilibrium state.
Directory of Open Access Journals (Sweden)
Tadashi Kawazoe
2014-01-01
Full Text Available We fabricated a high-efficiency infrared light emitting diode (LED via dressed-photon-phonon (DPP assisted annealing of a p-n homojunctioned bulk Si crystal. The center wavelength in the electroluminescence (EL spectrum of this LED was determined by the wavelength of a CW laser used in the DPP-assisted annealing. We have proposed a novel method of controlling the EL spectral shape by additionally using a pulsed light source in order to control the number of phonons for the DPP-assisted annealing. In this method, the Si crystal is irradiated with a pair of pulses having an arrival time difference between them. The number of coherent phonons created is increased (reduced by tuning (detuning this time difference. A Si-LED was subjected to DPP-assisted annealing using a 1.3 μm (hν=0.94 eV CW laser and a mode-locked pulsed laser with a pulse width of 17 fs. When the number of phonons was increased, the EL emission spectrum broadened toward the high-energy side by 200 meV or more. The broadening towards the low-energy side was reduced to 120 meV.
Effects of femtosecond laser radiation on the skin
Rogov, P. Yu; Bespalov, V. G.
2016-08-01
A mathematical model of linear and nonlinear processes is presented occurring under the influence of femtosecond laser radiation on the skin. There was held an analysis and the numerical solution of an equation system describing the dynamics of the electron and phonon subsystems were received. The results can be used to determine the maximum permissible levels of energy generated by femtosecond laser systems and the establishment of Russian laser safety standards for femtosecond laser systems.
Stefan, V. Alexander
2016-10-01
The ultraviolet photons may control the imbalance of sodium and potassium ions in the brain bioplasma and, consequently, may prove to be efficient in the prevention of epileptic seizures. A novel method is based on the multi-ultraviolet-photon beam interaction with the epilepsy-topion-bioplasma, (nonlinear coupling of an ultra high frequency mode to the brain beta phonons). It is hypothesized that epilepsy is a chaotic-dynamics phenomenon: small electrical changes in the epilepsy-topion-bioplasma lead, (within the 10s of milliseconds), to the onset of chaos, (seizure-excessive electrical discharge), and subsequent cascading into adjacent areas.
Scholz, Robert; Floß, Gereon; Saalfrank, Peter; Füchsel, Gernot; Lončarić, Ivor; Juaristi, J. I.
2016-10-01
A Langevin model accounting for all six molecular degrees of freedom is applied to femtosecond-laser induced, hot-electron driven dynamics of Ru(0001)(2 ×2 ):CO. In our molecular dynamics with electronic friction approach, a recently developed potential energy surface based on gradient-corrected density functional theory accounting for van der Waals interactions is adopted. Electronic friction due to the coupling of molecular degrees of freedom to electron-hole pairs in the metal are included via a local density friction approximation, and surface phonons by a generalized Langevin oscillator model. The action of ultrashort laser pulses enters through a substrate-mediated, hot-electron mechanism via a time-dependent electronic temperature (derived from a two-temperature model), causing random forces acting on the molecule. The model is applied to laser induced lateral diffusion of CO on the surface, "hot adsorbate" formation, and laser induced desorption. Reaction probabilities are strongly enhanced compared to purely thermal processes, both for diffusion and desorption. Reaction yields depend in a characteristic (nonlinear) fashion on the applied laser fluence, as well as branching ratios for various reaction channels. Computed two-pulse correlation traces for desorption and other indicators suggest that aside from electron-hole pairs, phonons play a non-negligible role for laser induced dynamics in this system, acting on a surprisingly short time scale. Our simulations on precomputed potentials allow for good statistics and the treatment of long-time dynamics (300 ps), giving insight into this system which hitherto has not been reached. We find generally good agreement with experimental data where available and make predictions in addition. A recently proposed laser induced population of physisorbed precursor states could not be observed with the present low-coverage model.
Multifunctional solid/solid phononic crystal
Swinteck, N.; Vasseur, J. O.; Hladky-Hennion, A. C.; Croënne, C.; Bringuier, S.; Deymier, P. A.
2012-07-01
A two-dimensional, solid/solid phononic crystal (PC) comprised a square array of steel cylinders in epoxy is shown to perform a variety of spectral, wave vector, and phase-space functions. Over a range of operating frequencies, the PC's elastic band structure shows uniquely shaped equifrequency contours that are only accessible to excitations of longitudinal polarization. Under this condition, the PC is shown to behave as (1) an acoustic wave collimator, (2) a defect-less wave guide, (3) a directional source for elastic waves, (4) an acoustic beam splitter, (5) a phase-control device, and (6) a k-space multiplexer. Wave vector diagrams and finite-difference time-domain simulations are employed to authenticate the above mentioned capabilities.
Phonon-Mediated Nonclassical Interference in Diamond
England, Duncan G.; Fisher, Kent A. G.; MacLean, Jean-Philippe W.; Bustard, Philip J.; Heshami, Khabat; Resch, Kevin J.; Sussman, Benjamin J.
2016-08-01
Quantum interference of single photons is a fundamental aspect of many photonic quantum processing and communication protocols. Interference requires that the multiple pathways through an interferometer be temporally indistinguishable to within the coherence time of the photon. In this Letter, we use a diamond quantum memory to demonstrate interference between quantum pathways, initially temporally separated by many multiples of the optical coherence time. The quantum memory can be viewed as a light-matter beam splitter, mapping a THz-bandwidth single photon to a variable superposition of the output optical mode and stored phononic mode. Because the memory acts both as a beam splitter and as a buffer, the relevant coherence time for interference is not that of the photon, but rather that of the memory. We use this mechanism to demonstrate nonclassical single-photon and two-photon interference between quantum pathways initially separated by several picoseconds, even though the duration of the photons themselves is just ˜250 fs .
Double Dirac cones in phononic crystals
Li, Yan
2014-07-07
A double Dirac cone is realized at the center of the Brillouin zone of a two-dimensional phononic crystal (PC) consisting of a triangular array of core-shell-structure cylinders in water. The double Dirac cone is induced by the accidental degeneracy of two double-degenerate Bloch states. Using a perturbation method, we demonstrate that the double Dirac cone is composed of two identical and overlapping Dirac cones whose linear slopes can also be accurately predicted from the method. Because the double Dirac cone occurs at a relatively low frequency, a slab of the PC can be mapped onto a slab of zero refractive index material by using a standard retrieval method. Total transmission without phase change and energy tunneling at the double Dirac point frequency are unambiguously demonstrated by two examples. Potential applications can be expected in diverse fields such as acoustic wave manipulations and energy flow control.
Geometrical tuning of thermal phonon spectrum in nanoribbons
Ramiere, Aymeric; Volz, Sebastian; Amrit, Jay
2016-03-01
Phonon spectral energy transmission in silicon nanoribbons is investigated using Monte-Carlo simulations in the boundary scattering regime by changing the length and width geometrical parameters. We show that the transition frequency from specular scattering to diffuse scattering is inversely proportional to the edge roughness σ with a geometry independent factor of proportionality. The increase of the length over width ratio \\zeta leads to a decrease of the energy transmission in the diffuse scattering regime which evolves as {{≤ft(1+{{\\zeta}0.59}\\right)}-1} . This trend is explained by developing a model of phonon energy transmission in the fully diffuse scattering regime which takes into account the probability for a diffusively scattered phonon to be directly transmitted from any position on the edge of the nanoribbon. This model establishes the importance of the solid angles in the energy transmission evolution with \\zeta . The transition from unity energy transmission in the specular scattering regime to reduced transmission in the diffuse scattering regime constitutes a low-pass frequency filter for phonons. Our simulations show an energy rejection rate better than 90% for high \\zeta , which paves the way for potential high performance filters. Filtering out high frequency phonons is of significant interest for phononic crystal applications, which use band engineering of phonons in the wave regime with low frequencies.
Single mode phonon energy transmission in functionalized carbon nanotubes.
Lee, Jonghoon; Varshney, Vikas; Roy, Ajit K; Farmer, Barry L
2011-09-14
Although the carbon nanotube (CNT) features superior thermal properties in its pristine form, the chemical functionalization often required for many applications of CNT inevitably degrades the structural integrity and affects the transport of energy carriers. In this article, the effect of the side wall functionalization on the phonon energy transmission along the symmetry axis of CNT is studied using the phonon wave packet method. Three different functional groups are studied: methyl (-CH(3)), vinyl (-C(2)H(3)), and carboxyl (-COOH). We find that, near Γ point of the Brillouin zone, acoustic phonons show ideal transmission, while the transmission of the optical phonons is strongly suppressed. A positive correlation between the energy transmission coefficient and the phonon group velocity is observed for both acoustic and optical phonon modes. On comparing the transmission due to functional groups with equivalent point mass defects on CNT, we find that the chemistry of the functional group, rather than its molecular mass, has a dominant role in determining phonon scattering, hence the transmission, at the defect sites.
Deterministic Single-Phonon Source Triggered by a Single Photon
Söllner, Immo; Lodahl, Peter
2016-01-01
We propose a scheme that enables the deterministic generation of single phonons at GHz frequencies triggered by single photons in the near infrared. This process is mediated by a quantum dot embedded on-chip in an opto-mechanical circuit, which allows for the simultaneous control of the relevant photonic and phononic frequencies. We devise new opto-mechanical circuit elements that constitute the necessary building blocks for the proposed scheme and are readily implementable within the current state-of-the-art of nano-fabrication. This will open new avenues for implementing quantum functionalities based on phonons as an on-chip quantum bus.
Phonon Quasidiffusion in Cryogenic Dark Matter Search Large Germanium Detectors
Leman, S W; McCarthy, K A; Pyle, M; Resch, R; Sadoulet, B; Sundqvist, K M; Brink, P L; Cherry, M; Silva, E Do Couto E; Figueroa-Feliciano, E; Mirabolfathi, N; Serfass, B; Tomada, A
2011-01-01
We present results on quasidiffusion studies in large, 3 inch diameter, 1 inch thick [100] high purity germanium crystals, cooled to 50 mK in the vacuum of a dilution refrigerator, and exposed with 59.5 keV gamma-rays from an Am-241 calibration source. We compare data obtained in two different detector types, with different phonon sensor area coverage, with results from a Monte Carlo. The Monte Carlo includes phonon quasidiffusion and the generation of phonons created by charge carriers as they are drifted across the detector by ionization readout channels.
Non-equilibrium phonon generation and detection in microstructure devices
Hertzberg, J. B.
2011-01-01
We demonstrate a method to excite locally a controllable, non-thermal distribution of acoustic phonon modes ranging from 0 to ∼200 GHz in a silicon microstructure, by decay of excited quasiparticle states in an attached superconducting tunnel junction (STJ). The phonons transiting the structure ballistically are detected by a second STJ, allowing comparison of direct with indirect transport pathways. This method may be applied to study how different phonon modes contribute to the thermal conductivity of nanostructures. © 2011 American Institute of Physics.
Decoherence in semiconductor cavity QED systems due to phonon couplings
DEFF Research Database (Denmark)
Nielsen, Per Kær; Mørk, Jesper
2014-01-01
We investigate the effect of electron-phonon interactions on the coherence properties of single photons emitted from a semiconductor cavity QED (quantum electrodynamics) system, i.e., a quantum dot embedded in an optical cavity. The degree of indistinguishability, governing the quantum mechanical...... interference between two single photons, is calculated as a function of important parameters describing the cavity QED system and the phonon reservoir, e.g., cavity quality factor, light-matter coupling strength, temperature, and phonon lifetime. We show that non-Markovian effects play an important role...
Bloch oscillations of THz acoustic phonons in coupled nanocavity structures.
Lanzillotti-Kimura, N D; Fainstein, A; Perrin, B; Jusserand, B; Mauguin, O; Largeau, L; Lemaître, A
2010-05-14
Nanophononic Bloch oscillations and Wannier-Stark ladders have been recently predicted to exist in specifically tailored structures formed by coupled nanocavities. Using pump-probe coherent phonon generation techniques we demonstrate that Bloch oscillations of terahertz acoustic phonons can be directly generated and probed in these complex nanostructures. In addition, by Fourier transforming the time traces we had access to the proper eigenmodes in the frequency domain, thus evidencing the related Wannier-Stark ladder. The observed Bloch oscillation dynamics are compared with simulations based on a model description of the coherent phonon generation and photoelastic detection processes.
PHONON SOFTENING IN INTERMEDIATE VALENT SmB6
Mörke, I.; Wachter, P.
1981-01-01
We have measured the Raman spectrum of a SmB6 single crystal and compared it to LaB6 and EuB6. Beside the three high energy Raman active phonons we found additional excitations in these compounds. Most prominent is a peak at 172 cm-1 for SmB6, 214 cm-1 for LaB6 and 220 cm-1 for EuB6. The spectra are analysed in terms of defect induced phonon scattering. The softening of the line in intermediate valent (IV) SmB6 is explained in analogy with the phonon anomalies found in other IV compounds.
The optical phonon spectrum of SmFeAsO
Marini, C.; Mirri, C.; Profeta, G.; Lupi, S.; Di Castro, D.; Sopracase, R.; Postorino, P.; Calvani, P.; Perucchi, A.; Massidda, S.; Tropeano, G. M.; Putti, M.; Martinelli, A.; Palenzona, A.; Dore, P.
2008-01-01
We measured the Raman and the Infrared phonon spectrum of SmFeAsO polycrystalline samples. We also performed Density Functional Theory calculations within the pseudopotential approximation to obtain the structural and dynamical lattice properties of both the SmFeAsO and the prototype LaFeAsO compounds. The measured Raman and Infrared phonon frequencies are well predicted by the optical phonon frequencies computed at the Gamma point, showing the capability of the employed ab-initio methods to ...
Quantum symmetries induced by phonons in the Hubbard model
Montorsi, Arianna; Rasetti, Mario
1994-03-01
We show how the addition of a phonon field to the Hubbard model deforms the superconducting su(2) part of the global symmetry Lie algebra su(2)⊗su(2)/openZ2, holding at half filling for the customary model, into a quantum [su(2)]q symmetry, holding for a filling which depends on the electron-phonon interaction strength. Such symmetry originates in the feature that in the presence of phonons the hopping amplitude turns out to depend on the coupling strength. The states generated by resorting to this q symmetry exhibit both off-diagonal long-range order and pairing.
Quantum symmetries induced by phonons in the Hubbard model
Montorsi, Arianna; Rasetti, Mario
1994-01-01
We show how the addition of a phonon field to the Hubbard model deforms the superconducting su(2) part of the global symmetry Lie algebra su(2)⊗su(2)/openZ2, holding at half filling for the customary model, into a quantum [su(2)]q symmetry, holding for a filling which depends on the electron-phonon interaction strength. Such symmetry originates in the feature that in the presence of phonons the hopping amplitude turns out to depend on the coupling strength. The states generated by resorting t...
Electron-phonon coupling in the rare-earth metals
DEFF Research Database (Denmark)
Skriver, Hans Lomholt; Mertig, I.
1990-01-01
We have estimated the strength of the mass enhancement of the conduction electrons due to electron-phonon interaction in the rare metals Sc, Y, and La–Lu. The underlying self-consistent energy bands were obtained by means of the scalar relativistic linear-muffin-tin-orbital method, and the electron......-phonon parameters were calculated within the Gaspari-Gyorffy formulation. For the heavier rare earths Gd–Tm spin polarization was included both in the band-structure calculations and in the treatment of the electron-phonon coupling to take into account the spin splitting of the conduction electrons induced by the 4...
Spin-seebeck effect: a phonon driven spin distribution.
Jaworski, C M; Yang, J; Mack, S; Awschalom, D D; Myers, R C; Heremans, J P
2011-05-06
Here we report on measurements of the spin-Seebeck effect in GaMnAs over an extended temperature range alongside the thermal conductivity, specific heat, magnetization, and thermoelectric power. The amplitude of the spin-Seebeck effect in GaMnAs scales with the thermal conductivity of the GaAs substrate and the phonon-drag contribution to the thermoelectric power of the GaMnAs, demonstrating that phonons drive the spin redistribution. A phenomenological model involving phonon-magnon drag explains the spatial and temperature dependence of the measured spin distribution.
Confined and interface phonons in combined cylindrical nanoheterosystem
Directory of Open Access Journals (Sweden)
O.M.Makhanets
2006-01-01
Full Text Available The spectra of all types of phonons existing in a complicated combined nanoheterosystem consisting of three cylindrical quantum dots embedded into the cylindrical quantum wire placed into vacuum are studied within the dielectric continuum model. It is shown that there are confined optical (LO and interface phonons of two types: top surface optical (TSO and side surface optical (SSO modes of vibration in such a nanosystem. The dependences of phonon energies on the quasiwave numbers and geometrical parameters of quantum dots are investigated and analysed.
Lifetimes of confined acoustic phonons in ultrathin silicon membranes.
Cuffe, J; Ristow, O; Chávez, E; Shchepetov, A; Chapuis, P-O; Alzina, F; Hettich, M; Prunnila, M; Ahopelto, J; Dekorsy, T; Sotomayor Torres, C M
2013-03-01
We study the relaxation of coherent acoustic phonon modes with frequencies up to 500 GHz in ultrathin free-standing silicon membranes. Using an ultrafast pump-probe technique of asynchronous optical sampling, we observe that the decay time of the first-order dilatational mode decreases significantly from ~4.7 ns to 5 ps with decreasing membrane thickness from ~194 to 8 nm. The experimental results are compared with theories considering both intrinsic phonon-phonon interactions and extrinsic surface roughness scattering including a wavelength-dependent specularity. Our results provide insight to understand some of the limits of nanomechanical resonators and thermal transport in nanostructures.
Research Update: Phonon engineering of nanocrystalline silicon thermoelectrics
Shiomi, Junichiro
2016-10-01
Nanocrystalline silicon thermoelectrics can be a solution to improve the cost-effectiveness of thermoelectric technology from both material and integration viewpoints. While their figure-of-merit is still developing, recent advances in theoretical/numerical calculations, property measurements, and structural synthesis/fabrication have opened up possibilities to develop the materials based on fundamental physics of phonon transport. Here, this is demonstrated by reviewing a series of works on nanocrystalline silicon materials using calculations of multiscale phonon transport, measurements of interfacial heat conduction, and synthesis from nanoparticles. Integration of these approaches allows us to engineer phonon transport to improve the thermoelectric performance by introducing local silicon-oxide structures.
Kamaraju, N.; Kumar, Sunil; Saha, Surajit; Singh, Surjeet; Suryanarayanan, R.; Revcolevschi, A.; Sood, A. K.
2011-04-01
We study the generation of coherent optical phonons in spin-frustrated pyrochlore single crystals Dy2Ti2O7, Gd2Ti2O7, and Tb2Ti2O7 using femtosecond laser pulses (65 fs, 1.57 eV) in degenerate time-resolved transmission experiments as a function of temperature from 4 to 296 K. At 4 K, two coherent phonons are observed at ~5.3 THz (5.0 THz) and ~9.3 THz (9.4 THz) for Dy2Ti2O7 (Gd2Ti2O7), whereas three coherent phonons are generated at ~5.0, 8.6, and 9.7 THz for Tb2Ti2O7. In the case of spin-ice Dy2Ti2O7, a clear discontinuity is observed in the linewidths of both the coherent phonons as well as in the phase of lower-energy coherent phonon mode, indicating a subtle structural change at 110 K. Another important observation is a phase difference of π between the modes in all the samples, thus suggesting that the driving forces behind the generation of these modes could be different in nature, unlike a purely impulsive or displacive mechanism.
Acoustic-optical phonon up-conversion and hot-phonon bottleneck in lead-halide perovskites
Yang, Jianfeng; Wen, Xiaoming; Xia, Hongze; Sheng, Rui; Ma, Qingshan; Kim, Jincheol; Tapping, Patrick; Harada, Takaaki; Kee, Tak W.; Huang, Fuzhi; Cheng, Yi-Bing; Green, Martin; Ho-Baillie, Anita; Huang, Shujuan; Shrestha, Santosh; Patterson, Robert; Conibeer, Gavin
2017-01-01
The hot-phonon bottleneck effect in lead-halide perovskites (APbX3) prolongs the cooling period of hot charge carriers, an effect that could be used in the next-generation photovoltaics devices. Using ultrafast optical characterization and first-principle calculations, four kinds of lead-halide perovskites (A=FA+/MA+/Cs+, X=I−/Br−) are compared in this study to reveal the carrier-phonon dynamics within. Here we show a stronger phonon bottleneck effect in hybrid perovskites than in their inorganic counterparts. Compared with the caesium-based system, a 10 times slower carrier-phonon relaxation rate is observed in FAPbI3. The up-conversion of low-energy phonons is proposed to be responsible for the bottleneck effect. The presence of organic cations introduces overlapping phonon branches and facilitates the up-transition of low-energy modes. The blocking of phonon propagation associated with an ultralow thermal conductivity of the material also increases the overall up-conversion efficiency. This result also suggests a new and general method for achieving long-lived hot carriers in materials. PMID:28106061
Acoustic-optical phonon up-conversion and hot-phonon bottleneck in lead-halide perovskites.
Yang, Jianfeng; Wen, Xiaoming; Xia, Hongze; Sheng, Rui; Ma, Qingshan; Kim, Jincheol; Tapping, Patrick; Harada, Takaaki; Kee, Tak W; Huang, Fuzhi; Cheng, Yi-Bing; Green, Martin; Ho-Baillie, Anita; Huang, Shujuan; Shrestha, Santosh; Patterson, Robert; Conibeer, Gavin
2017-01-20
The hot-phonon bottleneck effect in lead-halide perovskites (APbX3) prolongs the cooling period of hot charge carriers, an effect that could be used in the next-generation photovoltaics devices. Using ultrafast optical characterization and first-principle calculations, four kinds of lead-halide perovskites (A=FA(+)/MA(+)/Cs(+), X=I(-)/Br(-)) are compared in this study to reveal the carrier-phonon dynamics within. Here we show a stronger phonon bottleneck effect in hybrid perovskites than in their inorganic counterparts. Compared with the caesium-based system, a 10 times slower carrier-phonon relaxation rate is observed in FAPbI3. The up-conversion of low-energy phonons is proposed to be responsible for the bottleneck effect. The presence of organic cations introduces overlapping phonon branches and facilitates the up-transition of low-energy modes. The blocking of phonon propagation associated with an ultralow thermal conductivity of the material also increases the overall up-conversion efficiency. This result also suggests a new and general method for achieving long-lived hot carriers in materials.
Acoustic-optical phonon up-conversion and hot-phonon bottleneck in lead-halide perovskites
Yang, Jianfeng; Wen, Xiaoming; Xia, Hongze; Sheng, Rui; Ma, Qingshan; Kim, Jincheol; Tapping, Patrick; Harada, Takaaki; Kee, Tak W.; Huang, Fuzhi; Cheng, Yi-Bing; Green, Martin; Ho-Baillie, Anita; Huang, Shujuan; Shrestha, Santosh; Patterson, Robert; Conibeer, Gavin
2017-01-01
The hot-phonon bottleneck effect in lead-halide perovskites (APbX3) prolongs the cooling period of hot charge carriers, an effect that could be used in the next-generation photovoltaics devices. Using ultrafast optical characterization and first-principle calculations, four kinds of lead-halide perovskites (A=FA+/MA+/Cs+, X=I-/Br-) are compared in this study to reveal the carrier-phonon dynamics within. Here we show a stronger phonon bottleneck effect in hybrid perovskites than in their inorganic counterparts. Compared with the caesium-based system, a 10 times slower carrier-phonon relaxation rate is observed in FAPbI3. The up-conversion of low-energy phonons is proposed to be responsible for the bottleneck effect. The presence of organic cations introduces overlapping phonon branches and facilitates the up-transition of low-energy modes. The blocking of phonon propagation associated with an ultralow thermal conductivity of the material also increases the overall up-conversion efficiency. This result also suggests a new and general method for achieving long-lived hot carriers in materials.
Kuleev, I. I.; Bakharev, S. M.; Kuleev, I. G.; Ustinov, V. V.
2017-01-01
Effect of anisotropy of elastic energy on the phonon propagation in single-crystal nanowires made of Fe, Cu, MgO, InSb, and GaAs materials that are used to fabricate spintronics devices in the regime of the Knudsen flow of phonon gas has been studied. A new method of analyzing the focusing of quasi-transverse modes has been suggested, which made it possible to determine the average values of the densities of phonon states in the regions of focusing and defocusing slow and fast quasi-transverse modes. The effect of phonon focusing on the anisotropy of heat conductivity and lengths of the phonon free paths has been analyzed for all acoustic modes that exist in spintronics nanostructures. It has been shown that for all the nanowires investigated the angular dependences of the free paths of fast and slow transverse modes in the {100} and {110} planes correlate with the angular dependences of the densities of phonon states for these modes. Directions of the heat flux that ensure the maximum and minimum phonon heat conductivity in the nanowires have been determined.
Solution of the Boltzmann Equation for Electrons in Laser-Heated Metals
Pietanza, L. D.; Colonna, G.; Capitelli, M.
2005-05-01
A kinetic study of the electron relaxation dynamic inside a noble metal film (Ag) subjected to a femtosecond laser pulse has been performed. A time dependent numerical algorithm for the solution of the Boltzmann equations for electrons and phonons inside the film has been developped, considering electron-electron and electron-phonon collisions and the laser perturbation. The dependence of electron-electron and electron-phonon characteristic time-scales on the screening parameter values has been investigated. Electron-electron relaxation times are also compared with experimental data obtained through time-resolved two-photon photoemission technique.
Influence of anharmonic phonon decay on self-heating in Si nanowire transistors
Energy Technology Data Exchange (ETDEWEB)
Rhyner, Reto, E-mail: rhyner@iis.ee.ethz.ch; Luisier, Mathieu, E-mail: mluisier@iis.ee.ethz.ch [Integrated Systems Laboratory, ETH Zürich, Gloriastr. 35, 8092 Zürich (Switzerland)
2014-08-11
Anharmonic phonon-phonon scattering is incorporated into an electro-thermal quantum transport approach based on the nonequilibrium Green's function formalism. Electron-phonon and phonon-phonon interactions are taken into account through scattering self-energies solved in the self-consistent Born approximation. While studying self-heating effects in ultra-scaled Si nanowire transistors, it is found that the phonon decay process softens the artificial accumulation of high energy phonons caused by electron relaxations close to the drain region. This leads to an increase of the device current in the ON-state and a reduction of the effective lattice temperature.
Makovetskii, D N
2001-01-01
The microwave phonon stimulated emission (SE) has been experimentally and numerically investigated in a nonautonomous microwave acoustic quantum generator, called also microwave phonon laser or phaser (see previous works arXiv:cond-mat/0303188 ; arXiv:cond-mat/0402640 ; arXiv:nlin.CG/0703050) Phenomena of branching and long-time refractority (absence of the reaction on the external pulses) for deterministic chaotic and regular processes of SE were observed in experiments with various levels of electromagnetic pumping. At the pumping level growth, the clearly depined increasing of the number of coexisting SE states has been observed both in real physical experiments and in computer simulations. This confirms the analytical estimations of the branching density in the phase space. The nature of the refractority of SE pulses is closely connected with the pointed branching and reflects the crises of strange attractors, i.e. their collisions with unstable periodic components of the higher branches of SE states in t...
Phonon dispersion and electron-phonon coupling in MgB2 and AlB2.
Bohnen, K P; Heid, R; Renker, B
2001-06-18
We present a first principles investigation of the lattice dynamics and electron-phonon coupling of the superconductor MgB2 and the isostructural AlB2 within the framework of density functional perturbation theory using a mixed-basis pseudopotential method. Complete phonon dispersion curves and Eliashberg functions alpha2F are calculated for both systems. The main differences are related to high frequency in-plane boron vibrations, which are strongly softened in MgB2 and exhibit an exceptionally strong electron-phonon coupling. We also report on Raman measurements, which support the theoretical findings. Implications for the superconducting transition temperature are briefly discussed.
Indian Academy of Sciences (India)
B Ojha; P Nayak; S N Behera
2000-02-01
The electron–phonon interaction in the periodic Anderson model (PAM) is considered. The PAM incorporates the effect of onsite Coulomb interaction () between -electrons. The inﬂuence of Coulomb correlation on the phonon response of the system is studied by evaluating the phonon spectral function for various parameters of the model. The numerical evaluation of the spectral function is carried out in the long wavelength limit at ﬁnite temperatures keeping only linear terms in . The observed behaviour is found to agree well with the general features obtained experimentally for some heavy fermion (HF) systems.
The Electron-Phonon Interaction as Studied by Photoelectron Spectroscopy
Energy Technology Data Exchange (ETDEWEB)
D.W. Lynch
2004-09-30
With recent advances in energy and angle resolution, the effects of electron-phonon interactions are manifest in many valence-band photoelectron spectra (PES) for states near the Fermi level in metals.
Phonon transport in single-layer Boron nanoribbons
Zhang, Zhongwei; Peng, Qing; Chen, Yuanping
2016-01-01
Inspired by the successful synthesis of several allotropes, boron sheets have been one of the hottest spot areas of focus in various fields. Here, we study phonon transport in three types of boron nanoribbons with zigzag and armchair edges by using a non-equilibrium Green's function combined with first principles methods. Diverse transport properties are found in the nanoribbons. At the room temperature, their highest thermal conductance can be comparable with that of graphene, while the lowest thermal conductance is less than half of graphene's. The three boron sheets exhibit different anisotropic transport characteristics. Two of these sheets have stronger phonon transport abilities along the zigzag edges than the armchair edges, while in the case of the third, the results are reversed. With the analysis of phonon dispersion, bonding charge density, and simplified models of atomic chains, the mechanisms of the diverse phonon properties are discussed. Because all boron allotropes consists of hexagonal and tr...
Electron-phonon relaxation time in ultrathin tungsten silicon film
Sidorova, M; Korneev, A; Chulkova, G; Korneeva, Yu; Mikhailov, M; Devizenko, Yu; Kozorezov, A; Goltsman, G
2016-01-01
Using amplitude-modulated absorption of sub-THz radiation (AMAR) method, we studied electron-phonon relaxation in thin disordered films of tungsten silicide. We found a response time ~ 800 ps at critical temperature Tc = 3.4 K, which scales as minus 3 in the temperature range from 1.8 to 3.4 K. We discuss mechanisms, which can result in a strong phonon bottle-neck effect in a few nanometers thick film and yield a substantial difference between the measured time, characterizing response at modulation frequency, and the inelastic electron-phonon relaxation time. We estimate the electron-phonon relaxation time to be in the range ~ 100-200 ps at 3.4 K.
On the Cauchy Problem Describing an Electron-Phonon Interaction
Institute of Scientific and Technical Information of China (English)
Jo(a)o-Paulo DIAS; Mário FIGUEIRA; Filipe OLIVEIRA
2011-01-01
In this paper, a model is derived to describe a quartic anharmonic interatomic interaction with an external potential involving a pair electron-phonon. The authors study the corresponding Cauchy Problem in the semilinear and quasilinear cases.
Phonon-assisted decoherence and tunneling in quantum dot molecules
DEFF Research Database (Denmark)
Grodecka-Grad, Anna; Foerstner, Jens
2011-01-01
We study the influence of the phonon environment on the electron dynamics in a doped quantum dot molecule. A non-perturbative quantum kinetic theory based on correlation expansion is used in order to describe both diagonal and off-diagonal electron-phonon couplings representing real and virtual...... processes with relevant acoustic phonons. We show that the relaxation is dominated by phonon-assisted electron tunneling between constituent quantum dots and occurs on a picosecond time scale. The dependence of the time evolution of the quantum dot occupation probabilities on the energy mismatch between...... the quantum dots is studied in detail. (© 2011 WILEY-VCH Verlag GmbH & Co. KGaA, Weinheim)...
Influence of mass contrast in alloy phonon scattering
Shiga, Takuma; Shiomi, Junichiro
2015-01-01
We have investigated the effect of mass contrast on alloy phonon scattering in mass-substituted Lennard-Jones crystals. By calculating the mass-difference phonon scattering rate using a modal analysis method based on molecular dynamics, we have identified the applicability and limits of the widely-used mass-difference perturbation model in terms of magnitude and sign of the mass difference. The result of a phonon -mode-dependent analysis reveals that the critical phonon frequency, above which the mass-difference perturbation theory fails, decreases with the magnitude of the mass difference independently of its sign. This gives rise to a critical mass contrast, above which the mass-difference perturbation model noticeably underestimates the lattice thermal conductivity.
Flexural-Phonon Scattering Induced by Electrostatic Gating in Graphene
Gunst, Tue; Kaasbjerg, Kristen; Brandbyge, Mads
2017-01-01
Graphene has an extremely high carrier mobility partly due to its planar mirror symmetry inhibiting scattering by the highly occupied acoustic flexural phonons. Electrostatic gating of a graphene device can break the planar mirror symmetry, yielding a coupling mechanism to the flexural phonons. We examine the effect of the gate-induced one-phonon scattering on the mobility for several gate geometries and dielectric environments using first-principles calculations based on density functional theory and the Boltzmann equation. We demonstrate that this scattering mechanism can be a mobility-limiting factor, and show how the carrier density and temperature scaling of the mobility depends on the electrostatic environment. Our findings may explain the high deformation potential for in-plane acoustic phonons extracted from experiments and, furthermore, suggest a direct relation between device symmetry and resulting mobility.
Effect of pressure on the phonon properties of europium chalcogenides
Indian Academy of Sciences (India)
U K Sakalle; P K Jha; S P Sanyal
2000-06-01
Lattice vibrational properties of europium chalcogenides have been investigated at high pressure by using a simple lattice dynamical model theory viz. the three-body force rigid ion model (TRIM) which includes long range three-body interaction arising due to charge transfer effects. The dispersion curves for the four Eu-chalcogenides agree reasonably well with the available experimental data. Variation of LO, TO, LA and TA phonons with pressure have also been studied at the symmetry points of the brillouin zone (BZ) for Euchalcogenides for the first time by using a lattice dynamical model theory. We have also calculated the one phonon density of states and compared them with the first order Raman scattering results. The calculation of one phonon density of states for Eu-chalcogenides has also been extended up to the phase transition pressure. We observed a pronounced shift in phonon spectrum as pressure is increased.
Phonon Hall Effect in Four-Terminal Junctions
Zhang, Lifa; Wang, Jian-Sheng; Li, Baowen
2009-01-01
Using an exact nonequilibrium Green's function formulism, the phonon Hall effect for paramagnetic dielectrics is studied in a four-terminal device setting. The temperature difference in the transverse direction of the heat current is calculated for two-dimensional models with the magnetic field perpendicular to the plane. We find a surprising result that the square lattice does not have the phonon Hall effect while a honeycomb lattice has. This can be explained by symmetry. The temperature di...
Stochastic approach to phonon-assisted optical absorption
Zacharias, Marios; Patrick, Christopher E.; Giustino, Feliciano
2015-01-01
We develop a first-principles theory of phonon-assisted optical absorption in semiconductors and insulators which incorporates the temperature dependence of the electronic structure. We show that the Hall-Bardeen-Blatt theory of indirect optical absorption and the Allen-Heine theory of temperature-dependent band structures can be derived from the present formalism by retaining only one-phonon processes. We demonstrate this method by calculating the optical absorption coefficient of silicon us...
Far infrared absorption by acoustic phonons in titanium dioxide nanopowders
Murray, Daniel B.; Netting, Caleb H.; Saviot, Lucien; Pighini, Catherine; Millot, Nadine; Aymes, Daniel; Liu, Hsiang-Lin
2006-01-01
We report spectral features of far infrared electromagnetic radiation absorption in anatase TiO2 nanopowders which we attribute to absorption by acoustic phonon modes of nanoparticles. The frequency of peak excess absorption above the background level corresponds to the predicted frequency of the dipolar acoustic phonon from continuum elastic theory. The intensity of the absorption cannot be accounted for in a continuum elastic dielectric description of the nanoparticle material. Quantum mech...
Acoustic Bloch oscillations in a two-dimensional phononic crystal.
He, Zhaojian; Peng, Shasha; Cai, Feiyan; Ke, Manzhu; Liu, Zhengyou
2007-11-01
We report the observation of acoustic Bloch oscillations at megahertz frequency in a two-dimensional phononic crystal. By creating periodically arrayed cavities with a decreasing gradient in width along one direction in the phononic crystal, acoustic Wannier-Stark ladders are created in the frequency domain. The oscillatory motion of an incident Gaussian pulse inside the sample is demonstrated by both simulation and experiment.
On time-resolved approach for phonon assisted interband transitions
Klotins, E.
2015-03-01
Photoexcited dynamics of electrons and holes in two-band dielectric, with special emphasis on back reaction of phonons are developed by combining the quantum electrodynamics and Baker-Campbell-Hausdorff (BCH) canonical transformation. These methods create an explicit time-domain representation of photoinduced processes and contribute in unifying phonon-assisted description of distribution functions of electron and hole quasiparticles for the description of observable effects of photoinduced processes in dielectrics.
Experimental studies of electron-phonon interactions in gallium nitride
Stanton, N M
2001-01-01
This thesis presents an experimental investigation of the electron-phonon interaction in GaN. Bulk epilayers, grown by MBE, and AIGaN/GaN heterostructure grown by MOCVD, have been studied. The energy relaxation rate for hot electrons has been measured over a wide range of temperatures, allowing both acoustic and optic phonon emission to be studied in GaN epilayers. Direct phonon measurements, both studying the emission and absorption processes, have been performed. Detection of phonons emitted when hot electrons relax their excess energy complements the measurements of relaxation rates. Absorption of acoustic phonons by the epilayers, using both fixed and extended metal film phonon sources, allowed investigation into the effectiveness of the 2k sub F cutoff in the low mobility layers. The experimental findings are compared with the predictions of theory. AIGaN/GaN heterostructures were characterised and measurements of the energy relaxation rate in the temperature range 4K-40K obtained. Excellent agreement wi...
Polar phonon mixing in magnetoelectric EuTiO3
Goian, V.; Kamba, S.; Hlinka, J.; Vaněk, P.; Belik, A. A.; Kolodiazhnyi, T.; Petzelt, J.
2009-10-01
Infrared reflectivity spectra of antiferromagnetic incipient ferroelectric EuTiO3 were investigated up to 600 K. Three polar phonons typical for the cubic perovskite Pmbar {3}m structure were observed. Analysis of phonon plasma frequencies showed that the lowest-energy TO1 phonon corresponds predominantly to the Slater mode describing vibration of Ti cations against the oxygen octahedra and the TO2 phonon expresses vibrations of the Eu cation against the TiO6 octahedra. The highest frequency TO4 phonon represents O-octahedra bending. Incipient ferroelectric behavior of the permittivity is caused by pronounced softening of the TO1 phonon, which is coupled to the TO2 mode. Although the Eu cations are not involved in the TO1 mode, the spin ordering of the 4f electrons at Eu cations has influence on the frequency of the TO1 mode due to Eu-O-Eu super-exchange interaction. This is probably responsible for the 7% change of the permittivity induced by the magnetic field in the antiferromagnetic phase, as reported by Katsufuji and Takagi [Phys. Rev. B 64, 054415 (2001)].
Phonon anharmonicity and negative thermal expansion in SnSe
Bansal, Dipanshu; Hong, Jiawang; Li, Chen W.; May, Andrew F.; Porter, Wallace; Hu, Michael Y.; Abernathy, Douglas L.; Delaire, Olivier
2016-08-01
The anharmonic phonon properties of SnSe in the P n m a phase were investigated with a combination of experiments and first-principles simulations. Using inelastic neutron scattering (INS) and nuclear resonant inelastic X-ray scattering (NRIXS), we have measured the phonon dispersions and density of states (DOS) and their temperature dependence, which revealed a strong, inhomogeneous shift and broadening of the spectrum on warming. First-principles simulations were performed to rationalize these measurements, and to explain the previously reported anisotropic thermal expansion, in particular the negative thermal expansion within the Sn-Se bilayers. Including the anisotropic strain dependence of the phonon free energy, in addition to the electronic ground state energy, is essential to reproduce the negative thermal expansion. From the phonon DOS obtained with INS and additional calorimetry measurements, we quantify the harmonic, dilational, and anharmonic components of the phonon entropy, heat capacity, and free energy. The origin of the anharmonic phonon thermodynamics is linked to the electronic structure.
Decomposition model for phonon thermal conductivity of a monatomic lattice
Evteev, Alexander V.; Momenzadeh, Leila; Levchenko, Elena V.; Belova, Irina V.; Murch, Graeme E.
2014-12-01
An analytical treatment of decomposition of the phonon thermal conductivity of a crystal with a monatomic unit cell is developed on the basis of a two-stage decay of the heat current autocorrelation function observed in molecular dynamics simulations. It is demonstrated that the contributions from the acoustic short- and long-range phonon modes to the total phonon thermal conductivity can be presented in the form of simple kinetic formulas, consisting of products of the heat capacity and the average relaxation time of the considered phonon modes as well as the square of the average phonon velocity. On the basis of molecular dynamics calculations of the heat current autocorrelation function, this treatment allows for a self-consistent numerical evaluation of the aforementioned variables. In addition, the presented analysis allows, within the Debye approximation, for the identification of the temperature range where classical molecular dynamics simulations can be employed for the prediction of phonon thermal transport properties. As a case example, Cu is considered.
Coupling of Excitons and Discrete Acoustic Phonons in Vibrationally Isolated Quantum Emitters.
Werschler, Florian; Hinz, Christopher; Froning, Florian; Gumbsheimer, Pascal; Haase, Johannes; Negele, Carla; de Roo, Tjaard; Mecking, Stefan; Leitenstorfer, Alfred; Seletskiy, Denis V
2016-09-14
The photoluminescence emission by mesoscopic condensed matter is ultimately dictated by the fine-structure splitting of the fundamental exciton into optically allowed and dipole-forbidden states. In epitaxially grown semiconductor quantum dots, nonradiative equilibration between the fine-structure levels is mediated by bulk acoustic phonons, resulting in asymmetric spectral broadening of the excitonic luminescence. In isolated colloidal quantum dots, spatial confinement of the vibrational motion is expected to give rise to an interplay between the quantized electronic and phononic degrees of freedom. In most cases, however, zero-dimensional colloidal nanocrystals are strongly coupled to the substrate such that the charge relaxation processes are still effectively governed by the bulk properties. Here we show that encapsulation of single colloidal CdSe/CdS nanocrystals into individual organic polymer shells allows for systematic vibrational decoupling of the semiconductor nanospheres from the surroundings. In contrast to epitaxially grown quantum dots, simultaneous quantization of both electronic and vibrational degrees of freedom results in a series of strong and narrow acoustic phonon sidebands observed in the photoluminescence. Furthermore, an individual analysis of more than 200 compound particles reveals that enhancement or suppression of the radiative properties of the fundamental exciton is controlled by the interaction between fine-structure states via the discrete vibrational modes. For the first time, pronounced resonances in the scattering rate between the fine-structure states are directly observed, in good agreement with a quantum mechanical model. The unambiguous assignment of mediating acoustic modes to the observed scattering resonances complements the experimental findings. Thus, our results form an attractive basis for future studies on subterahertz quantum opto-mechanics and efficient laser cooling at the nanoscale.
Mesoscopic hydro-thermodynamics of phonons
Directory of Open Access Journals (Sweden)
Aurea R. Vasconcellos
2013-07-01
Full Text Available A generalized Hydrodynamics, referred to as Mesoscopic Hydro-Thermodynamics, of phonons in semiconductors is presented. It involves the descriptions of the motion of the quasi-particle density and of the energy density. The hydrodynamic equations, which couple both types of movement via thermo-elastic processes, are derived starting with a generalized Peierls-Boltzmann kinetic equation obtained in the framework of a Non-Equilibrium Statistical Ensemble Formalism, providing such Mesoscopic Hydro-Thermodynamics. The case of a contraction in first order is worked out in detail. The associated Maxwell times are derived and discussed. The densities of quasi-particles and of energy are found to satisfy coupled Maxwell-Cattaneo-like (hyperbolic equations. The analysis of thermo-elastic effects is done and applied to investigate thermal distortion in silicon mirrors under incidence of high intensity X-ray pulses in FEL facilities. The derivation of a generalized Guyer-Krumhansl equation governing the flux of heat and the associated thermal conductivity coefficient is also presented.
TOPICAL REVIEW: Photonic and phononic quasicrystals
Steurer, Walter; Sutter-Widmer, Daniel
2007-07-01
This review focuses on the peculiarities of quasiperiodic order for the properties of photonic and phononic (sonic) heterostructures. The most beneficial feature of quasiperiodicity is that it can combine perfectly ordered structures with purely point-diffractive spectra of arbitrarily high rotational symmetry. Both are prerequisites for the construction of isotropic band gap composites, in particular from materials with low index contrast, which are required for numerous applications. Another interesting property of quasiperiodic structures is their scaling symmetry, which may be exploited to create spectral gaps in the sub-wavelength regime. This review covers structure/property relationships of heterostructures based on one-dimensional (1D) substitutional sequences such as the Fibonacci, Thue Morse, period-doubling, Rudin Shapiro and Cantor sequence as well as on 1D modulated structures, further on 2D tilings with 8-, 10-, 12- and 14-fold symmetry as well as on the pinwheel tiling, the Sierpinski gasket and on curvilinear tilings and, finally, on the 3D icosahedral Penrose tiling.
Polarization dependent behavior of CdS around the first and second LO-phonon modes
Energy Technology Data Exchange (ETDEWEB)
Frausto-Reyes, C., E-mail: cfraus@cio.mx [Centro de Investigaciones en Optica AC, Unidad Aguascalientes, Prolong., Constitucion 607, Fracc. Reserva Loma Bonita, CP 20200, Apartado Postal 507, Ags. (Mexico); Molina-Contreras, J.R., E-mail: rmolina@correo.ita.mx [Departamento de Ingenieria Electrica y Electronica, Instituto Tecnologico de Aguascalientes, Av. Lopez Mateos 1081 Oriente, Fracc. Bonna Gens, CP 20256, Aguascalientes, Ags. (Mexico); Lopez-Alvarez, Y.F. [Departamento de Ingenieria Electrica y Electronica, Instituto Tecnologico de Aguascalientes, Av. Lopez Mateos 1081 Oriente, Fracc. Bonna Gens, CP 20256, Aguascalientes, Ags. (Mexico); Medel-Ruiz, C.I.; Perez Ladron de Guevara, H. [Universidad de Guadalajara, Centro Universitario de los Lagos, Av. Enrique Diaz de Leon s/n, Fracc. Paseos de la Montana, CP 47460, Lagos de Moreno, Jal. (Mexico); Ortiz-Morales, M. [Centro de Investigaciones en Optica AC, Unidad Aguascalientes, Prolong., Constitucion 607, Fracc. Reserva Loma Bonita, CP 20200, Apartado Postal 507, Ags. (Mexico)
2010-10-25
The present work report studies on resonant Raman experimental line shape for CdS around the first and second LO-phonon modes. The application of our method to the study of LO-phonon modes of CdS suggests that the scattered intensity is dominated by the surface and dependent on polarization. Results showed that the Raman spectra for CdS, roughly fall into three groups: a broad line-wing with apparent maxima around 194 cm{sup -1} in the range of 140 and 240 cm{sup -1} which can be ascribed to overtone scattering from acoustic phonons; a band near the 1LO phonon mode which can be attributed to a combination of one-phonon scattering and peak acoustic phonon and finally, a band near the 2LO phonon mode which can be attributed to a combination of two-phonon scattering and peak acoustic phonon.
Energy Technology Data Exchange (ETDEWEB)
Kityk, I.V. [Institute of Physics, J. Dlugosz University Czestochowa, Al. Armii Krajowej 13/15, Czestochowa (Poland)]. E-mail: i.kityk@ajd.czest.pl; Guignard, M. [UMR CNRS 6226 Sciences Chimiques de Rennes, Universite de Rennes 1, 35000 Rennes (France); Nazabal, V. [UMR CNRS 6226 Sciences Chimiques de Rennes, Universite de Rennes 1, 35000 Rennes (France); Zhang, X.H. [UMR CNRS 6226 Sciences Chimiques de Rennes, Universite de Rennes 1, 35000 Rennes (France); Troles, J. [UMR CNRS 6226 Sciences Chimiques de Rennes, Universite de Rennes 1, 35000 Rennes (France); Smektala, F. [UMR CNRS 6226 Sciences Chimiques de Rennes, Universite de Rennes 1, 35000 Rennes (France); Sahraoui, B. [Laboratoire POMA, Universite d' Angers Bld. Lavouisier 2, Angers, UMR CNRS 6136 (France); Boudebs, G. [Laboratoire POMA, Universite d' Angers Bld. Lavouisier 2, Angers, UMR CNRS 6136 (France)
2007-04-01
The non-linear optical response of sulphide glass-containing {beta}-GeS{sub 2} microcrystallites, has been studied at a fundamental wavelength of {lambda}=5.5 {mu}m under additional irradiation by IR-pulses of {lambda}=3.7 {mu}m. A substantial increase of the non-linear susceptibility with IR-power and size of the microcrystallites has been found. Molecular dynamics calculations linked to quantum chemical calculations show that this effect could be explained by substantial contributions of the microcrystallite interfaces and due to the phonon sub-system. The role of anharmonic electron-phonon effects is experimentally confirmed by the observation of an optimal delay of 8 ps between the pump laser pulses at 3.7 {mu}m and the probing laser pulses at 5.5 {mu}m, which generate the observed second harmonic signal.
Thermal characterization of nanoscale phononic crystals using supercell lattice dynamics
Directory of Open Access Journals (Sweden)
Bruce L. Davis
2011-12-01
Full Text Available The concept of a phononic crystal can in principle be realized at the nanoscale whenever the conditions for coherent phonon transport exist. Under such conditions, the dispersion characteristics of both the constitutive material lattice (defined by a primitive cell and the phononic crystal lattice (defined by a supercell contribute to the value of the thermal conductivity. It is therefore necessary in this emerging class of phononic materials to treat the lattice dynamics at both periodicity levels. Here we demonstrate the utility of using supercell lattice dynamics to investigate the thermal transport behavior of three-dimensional nanoscale phononic crystals formed from silicon and cubic voids of vacuum. The periodicity of the voids follows a simple cubic arrangement with a lattice constant that is around an order of magnitude larger than that of the bulk crystalline silicon primitive cell. We consider an atomic-scale supercell which incorporates all the details of the silicon atomic locations and the void geometry. For this supercell, we compute the phonon band structure and subsequently predict the thermal conductivity following the Callaway-Holland model. Our findings dictate that for an analysis based on supercell lattice dynamics to be representative of the properties of the underlying lattice model, a minimum supercell size is needed along with a minimum wave vector sampling resolution. Below these minimum values, a thermal conductivity prediction of a bulk material based on a supercell will not adequately recover the value obtained based on a primitive cell. Furthermore, our results show that for the relatively small voids and void spacings we consider (where boundary scattering is dominant, dispersion at the phononic crystal unit cell level plays a noticeable role in determining the thermal conductivity.
Thermal characterization of nanoscale phononic crystals using supercell lattice dynamics
Davis, Bruce L.; Hussein, Mahmoud I.
2011-12-01
The concept of a phononic crystal can in principle be realized at the nanoscale whenever the conditions for coherent phonon transport exist. Under such conditions, the dispersion characteristics of both the constitutive material lattice (defined by a primitive cell) and the phononic crystal lattice (defined by a supercell) contribute to the value of the thermal conductivity. It is therefore necessary in this emerging class of phononic materials to treat the lattice dynamics at both periodicity levels. Here we demonstrate the utility of using supercell lattice dynamics to investigate the thermal transport behavior of three-dimensional nanoscale phononic crystals formed from silicon and cubic voids of vacuum. The periodicity of the voids follows a simple cubic arrangement with a lattice constant that is around an order of magnitude larger than that of the bulk crystalline silicon primitive cell. We consider an atomic-scale supercell which incorporates all the details of the silicon atomic locations and the void geometry. For this supercell, we compute the phonon band structure and subsequently predict the thermal conductivity following the Callaway-Holland model. Our findings dictate that for an analysis based on supercell lattice dynamics to be representative of the properties of the underlying lattice model, a minimum supercell size is needed along with a minimum wave vector sampling resolution. Below these minimum values, a thermal conductivity prediction of a bulk material based on a supercell will not adequately recover the value obtained based on a primitive cell. Furthermore, our results show that for the relatively small voids and void spacings we consider (where boundary scattering is dominant), dispersion at the phononic crystal unit cell level plays a noticeable role in determining the thermal conductivity.
Temperature dependent magnon-phonon coupling in bcc Fe from theory and experiment.
Körmann, F; Grabowski, B; Dutta, B; Hickel, T; Mauger, L; Fultz, B; Neugebauer, J
2014-10-17
An ab initio based framework for quantitatively assessing the phonon contribution due to magnon-phonon interactions and lattice expansion is developed. The theoretical results for bcc Fe are in very good agreement with high-quality phonon frequency measurements. For some phonon branches, the magnon-phonon interaction is an order of magnitude larger than the phonon shift due to lattice expansion, demonstrating the strong impact of magnetic short-range order even significantly above the Curie temperature. The framework closes the previous simulation gap between the ferro- and paramagnetic limits.
Phonon transport in perovskite SrTiO3 from first principles
Feng, Lei; Shiomi, Junichiro
2015-01-01
We investigate phonon transport in perovskite strontium titanate (SrTiO3) which is stable above its phase transition temperature (~105 K) by using first-principles molecular dynamics and anharmonic lattice dynamics. Unlike conventional ground-state-based perturbation methods that give imaginary phonon frequencies, the current calculation reproduces stable phonon dispersion relations observed in experiments. We find the contribution of optical phonons to overall lattice thermal conductivity is larger than 60%, markedly different from the usual picture with dominant contribution from acoustic phonons. The mode- and pseudopotential-dependence analysis suggests the strong attenuation of acoustic phonons transport originated from strong anharmonic coupling with the transversely-polarized ferroelectric modes.
Laser cooling and control of excitations in superfluid helium
Harris, G. I.; McAuslan, D. L.; Sheridan, E.; Sachkou, Y.; Baker, C.; Bowen, W. P.
2016-08-01
Superfluidity is a quantum state of matter that exists macroscopically in helium at low temperatures. The elementary excitations in superfluid helium have been probed with great success using techniques such as neutron and light scattering. However, measurements of phonon excitations have so far been limited to average thermodynamic properties or the driven response far out of thermal equilibrium. Here, we use cavity optomechanics to probe the thermodynamics of phonon excitations in real time. Furthermore, strong light-matter interactions allow both laser cooling and amplification. This represents a new tool to observe and control superfluid excitations that may provide insight into phonon-phonon interactions, quantized vortices and two-dimensional phenomena such as the Berezinskii-Kosterlitz-Thouless transition. The third sound modes studied here also offer a pathway towards quantum optomechanics with thin superfluid films, including the prospect of femtogram masses, high mechanical quality factors, strong phonon-phonon and phonon-vortex interactions, and self-assembly into complex geometries with sub-nanometre feature size.
Acoustic phonon dynamics in thin-films of the topological insulator Bi{sub 2}Se{sub 3}
Energy Technology Data Exchange (ETDEWEB)
Glinka, Yuri D., E-mail: ydglinka@mail.wvu.edu [Department of Physics and Astronomy, West Virginia University, Morgantown, West Virginia 26506-6315 (United States); Institute of Physics, National Academy of Sciences of Ukraine, Kiev 03028 (Ukraine); Babakiray, Sercan; Johnson, Trent A.; Holcomb, Mikel B.; Lederman, David [Department of Physics and Astronomy, West Virginia University, Morgantown, West Virginia 26506-6315 (United States)
2015-04-28
Transient reflectivity traces measured for nanometer-sized films (6–40 nm) of the topological insulator Bi{sub 2}Se{sub 3} revealed GHz-range oscillations driven within the relaxation of hot carriers photoexcited with ultrashort (∼100 fs) laser pulses of 1.51 eV photon energy. These oscillations have been suggested to result from acoustic phonon dynamics, including coherent longitudinal acoustic phonons in the form of standing acoustic waves. An increase of oscillation frequency from ∼35 to ∼70 GHz with decreasing film thickness from 40 to 15 nm was attributed to the interplay between two different regimes employing traveling-acoustic-waves for films thicker than 40 nm and the film bulk acoustic wave resonator (FBAWR) modes for films thinner than 40 nm. The amplitude of oscillations decays rapidly for films below 15 nm thick when the indirect intersurface coupling in Bi{sub 2}Se{sub 3} films switches the FBAWR regime to that of the Lamb wave excitation. The frequency range of coherent longitudinal acoustic phonons is in good agreement with elastic properties of Bi{sub 2}Se{sub 3}.
Institute of Scientific and Technical Information of China (English)
ZHANG Li
2011-01-01
Within the framework of the macroscopic dielectric continuum model and Loudon's uniaxial crystal model,the phonon modes of a wurtzite/zinc-blende one-dimensional (ID) cylindrical nanowire (NW) are derived and studied.The analytical phonon states of phonon modes are given.It is found that there exist two types of polar phonon modes,i.e.interface optical (IO) phonon modes and the quasi-confined (QC) phonon modes existing in 1D wurtzite/zinc-blende NWs.Via the standard procedure of field quantization, the Frohlich electron-phonon interaction Hamiltonians are obtained.Numerical calculations of dispersive behavior of these phonon modes on a wurtzite/zinc-blende ZnO/MgO NW are performed.The frequency ranges of the I0 and QC phonon modes of the ZnO/MgO NWs are analyzed and discussed.It is found that the IO modes only exist in one frequency range, while QC modes may appear in three frequency ranges.The dispersive properties of the IO and QC modes on the free wave-number kz and the azimuthal quantum number m are discussed.The analytical Hamiltonians of electron-phonon interaction obtained here are quite useful for further investigating phonon influence on optoelectronics properties of wurtzite/zinc-blende 1D NW structures.
Hoffmann, Stanislaw K.; Lijewski, Stefan
2015-03-01
Electron spin-lattice relaxation rate is determined by electron spin echo method in temperature range 4-60 K. The Raman relaxation processes dominate and its theory is outlined in a form suitable for calculations of relaxation rate using real phonon spectrum. A few approximations have been considered: when phonon spectrum and Debye temperature are not available; when Debye temperature is available but phonon spectrum is not; and when spin-phonon coupling is known. All these approximations use the Debye model of phonons and give a non-satisfactory description the temperature dependence of the relaxation rate. A perfect description of experimental results is obtained when real phonon spectrum is considered. The value of the spin-phonon coupling parameter was determined as G = = 1362cm-1 . This value is discussed by a comparison with G-values published for various ions and crystals.
Xu, Zhi-Jie
2015-01-01
We first propose fundamental solutions of wave propagation in dispersive chain subject to a localized initial perturbation in the displacement. Analytical solutions are obtained for both second order nonlinear dispersive chain and homogenous harmonic chain using stationary phase approximation. Solution is also compared with numerical results from molecular dynamics (MD) simulations. Locally dominant phonon modes (k-space) are introduced based on these solutions. These locally defined spatially and temporally varying phonon modes k(x, t) are critical to the concept of the local thermodynamic equilibrium (LTE). Wave propagation accompanying with the nonequilibrium dynamics leads to the excitation of these locally defined phonon modes. It is found that the system energy is gradually redistributed among these excited phonons modes (k-space). This redistribution process is only possible with nonlinear dispersion and requires a finite amount of time to achieve a steady state distribution. This time scale is dependent on the spatial distribution (or frequency content) of the initial perturbation and the dispersion relation. Sharper and more concentrated perturbation leads to a faster energy redistribution and dissipation. This energy redistribution generates localized phonons with various frequencies that can be important for phonon-phonon interaction and energy dissipation in nonlinear systems. Depending on the initial perturbation and temperature, the time scale associated with this energy distribution can be critical for energy dissipation compared to the Umklapp scattering process. Ballistic type of heat transport along the harmonic chain reveals that at any given position, the lowest mode (k = 0) is excited first and gradually expanding to the highest mode (kmax(x,t)), where kmax(x,t) can only asymptotically approach the maximum mode kB of the first Brillouin zone (kmax(x,t) → kB). No energy distributed into modes with kmax(x,t) proportional to the sound speed
Reduction of thermal conductivity in phononic nanomesh structures
Yu, Jen-Kan
2010-07-25
Controlling the thermal conductivity of a material independently of its electrical conductivity continues to be a goal for researchers working on thermoelectric materials for use in energy applications1,2 and in the cooling of integrated circuits3. In principle, the thermal conductivity κ and the electrical conductivity σ may be independently optimized in semiconducting nanostructures because different length scales are associated with phonons (which carry heat) and electric charges (which carry current). Phonons are scattered at surfaces and interfaces, so κ generally decreases as the surface-to-volume ratio increases. In contrast, σ is less sensitive to a decrease in nanostructure size, although at sufficiently small sizes it will degrade through the scattering of charge carriers at interfaces. Here, we demonstrate an approach to independently controlling κ based on altering the phonon band structure of a semiconductor thin film through the formation of a phononic nanomesh film. These films are patterned with periodic spacings that are comparable to, or shorter than, the phonon mean free path. The nanomesh structure exhibits a substantially lower thermal conductivity than an equivalently prepared array of silicon nanowires, even though this array has a significantly higher surface-to-volume ratio. Bulk-like electrical conductivity is preserved. We suggest that this development is a step towards a coherent mechanism for lowering thermal conductivity. © 2010 Macmillan Publishers Limited. All rights reserved.
Functional crossover in the dispersion relations of magnons and phonons
Hoser, A.; Köbler, U.
2016-09-01
Experimental data are presented showing that the dispersion relations of magnons and acoustic phonons can consist of two sections with different functions of wave vector. In the low wave vector range a power function of wave vector often holds over a finite q-range while dispersions for larger wave vector values better approach the atomistic model predictions. In the magnon spectra ∼⃒qx power functions with exponents x=1.25, 1.5 and 2 are identified. The dispersion of the acoustic phonons can be a linear function of wave vector over a surprisingly large range of energy. Since the slope of the linear section agrees with the known sound velocities it can be concluded that the dispersion of the acoustic phonons has got attracted by the linear dispersion of the mass less Debye bosons (sound waves). Due to the different (translational) symmetries of bosons and atomistic excitations (magnons, phonons) the associated dispersions can attract each other. In the same way the different ∼⃒qx power functions in the magnon dispersions indicate that magnon dispersions are attracted by the dispersion of the bosons of the magnetic continuum (Goldstone bosons). This allows evaluation of the otherwise difficult to obtain dispersions of the Goldstone bosons from the known magnon dispersions. Interestingly, the dispersions of Goldstone bosons (Debye bosons) attract magnon dispersions (phonon dispersions) and not vice versa.
Investigation of phonon coherence and backscattering using silicon nanomeshes
Lee, Jaeho; Lee, Woochul; Wehmeyer, Geoff; Dhuey, Scott; Olynick, Deirdre L.; Cabrini, Stefano; Dames, Chris; Urban, Jeffrey J.; Yang, Peidong
2017-01-01
Phonons can display both wave-like and particle-like behaviour during thermal transport. While thermal transport in silicon nanomeshes has been previously interpreted by phonon wave effects due to interference with periodic structures, as well as phonon particle effects including backscattering, the dominant mechanism responsible for thermal conductivity reductions below classical predictions still remains unclear. Here we isolate the wave-related coherence effects by comparing periodic and aperiodic nanomeshes, and quantify the backscattering effect by comparing variable-pitch nanomeshes. We measure identical (within 6% uncertainty) thermal conductivities for periodic and aperiodic nanomeshes of the same average pitch, and reduced thermal conductivities for nanomeshes with smaller pitches. Ray tracing simulations support the measurement results. We conclude phonon coherence is unimportant for thermal transport in silicon nanomeshes with periodicities of 100 nm and higher and temperatures above 14 K, and phonon backscattering, as manifested in the classical size effect, is responsible for the thermal conductivity reduction. PMID:28051081
Thermally triggered phononic gaps in liquids at THz scale
Bolmatov, Dima; Zhernenkov, Mikhail; Zav'Yalov, Dmitry; Stoupin, Stanislav; Cunsolo, Alessandro; Cai, Yong Q.
2016-01-01
In this paper we present inelastic X-ray scattering experiments in a diamond anvil cell and molecular dynamic simulations to investigate the behavior of phononic excitations in liquid Ar. The spectra calculated using molecular dynamics were found to be in a good agreement with the experimental data. Furthermore, we observe that, upon temperature increases, a low-frequency transverse phononic gap emerges while high-frequency propagating modes become evanescent at the THz scale. The effect of strong localization of a longitudinal phononic mode in the supercritical phase is observed for the first time. The evidence for the high-frequency transverse phononic gap due to the transition from an oscillatory to a ballistic dynamic regimes of motion is presented and supported by molecular dynamics simulations. This transition takes place across the Frenkel line thermodynamic limit which demarcates compressed liquid and non-compressed fluid domains on the phase diagram and is supported by calculations within the Green-Kubo phenomenological formalism. These results are crucial to advance the development of novel terahertz thermal devices, phononic lenses, mirrors, and other THz metamaterials.
Energy Technology Data Exchange (ETDEWEB)
Flach, B.
2000-01-01
This thesis has two topics: One is the investigation of an adsorbate induced phonon anomaly on W(110) and Mo{sub 1-x}Re{sub x}(110) (x = 5, 15, 25%) with inelastic helium atom scattering (HAS). The other one is the study of the growth, morphology and dynamics of ultra-thin lithium films deposited on W(110). In 1992 a giant phonon anomaly was found by J. Luedecke on the hydrogen saturated W(110) and Mo(110) surfaces. The anomaly consists of a deep and sharp indentation in the phonon dispersion curves in which the phonon energy nearly drops to zero ({omega}{sub 1}). In addition, a small and broad dip in the surface Rayleigh mode is observed ({omega}{sub 2}). The anomaly appears in the anti {gamma}-H- as well as in the anti {gamma}-S-direction of the surface Brillouin zone (SBZ). Since its first discovery, numerous other experimental and theoretical studies have followed. In the present work the effects is reinvestigated and experimental parameters, such as the crystal temperature and the incident energy, were changed in order to study their influence on the anomalous phonon behavior. In the case of H/Mo(110) the substrate was changed as well by alloying with small amounts of rhenium. In the present experiments a strong crystal temperature dependence of the {omega}{sub 2}-branch was found which leads to lower energies at the 'dip' for smaller temperatures, while the {omega}{sub 1}-anomaly remains unchanged. Such behavior agrees well with the picture that the {omega}{sub 2}-branch is due to a Kohn anomaly. (orig.)
Giles, Alexander J; Dai, Siyuan; Glembocki, Orest J; Kretinin, Andrey V; Sun, Zhiyuan; Ellis, Chase T; Tischler, Joseph G; Taniguchi, Takashi; Watanabe, Kenji; Fogler, Michael M; Novoselov, Kostya S; Basov, Dimitri N; Caldwell, Joshua D
2016-06-08
We use scanning near-field optical microscopy to study the response of hexagonal boron nitride nanocones at infrared frequencies, where this material behaves as a hyperbolic medium. The obtained images are dominated by a series of "hot" rings that occur on the sloped sidewalls of the nanocones. The ring positions depend on the incident laser frequency and the nanocone shape. Both dependences are consistent with directional propagation of hyperbolic phonon-polariton rays that are launched at the edges and zigzag through the interior of the nanocones, sustaining multiple internal reflections off the sidewalls. Additionally, we observe a strong overall enhancement of the near-field signal at discrete resonance frequencies. These resonances attest to low dielectric losses that permit coherent standing waves of the subdiffractional polaritons to form. We comment on potential applications of such shape-dependent resonances and the field concentration at the hot rings.
Nardi, Damiano; Travagliati, Marco; Siemens, Mark E; Li, Qing; Murnane, Margaret M; Kapteyn, Henry C; Ferrini, Gabriele; Parmigiani, Fulvio; Banfi, Francesco
2011-10-12
High-frequency surface acoustic waves can be generated by ultrafast laser excitation of nanoscale patterned surfaces. Here we study this phenomenon in the hypersonic frequency limit. By modeling the thermomechanics from first-principles, we calculate the system's initial heat-driven impulsive response and follow its time evolution. A scheme is introduced to quantitatively access frequencies and lifetimes of the composite system's excited eigenmodes. A spectral decomposition of the calculated response on the eigemodes of the system reveals asymmetric resonances that result from the coupling between surface and bulk acoustic modes. This finding allows evaluation of impulsively excited pseudosurface acoustic wave frequencies and lifetimes and expands our understanding of the scattering of surface waves in mesoscale metamaterials. The model is successfully benchmarked against time-resolved optical diffraction measurements performed on one-dimensional and two-dimensional surface phononic crystals, probed using light at extreme ultraviolet and near-infrared wavelengths.
Theory and experimental evidence of phonon domains and their roles in pre-martensitic phenomena
Jin, Yongmei M.; Wang, Yu U.; Ren, Yang
2015-12-01
Pre-martensitic phenomena, also called martensite precursor effects, have been known for decades while yet remain outstanding issues. This paper addresses pre-martensitic phenomena from new theoretical and experimental perspectives. A statistical mechanics-based Grüneisen-type phonon theory is developed. On the basis of deformation-dependent incompletely softened low-energy phonons, the theory predicts a lattice instability and pre-martensitic transition into elastic-phonon domains via 'phonon spinodal decomposition.' The phase transition lifts phonon degeneracy in cubic crystal and has a nature of phonon pseudo-Jahn-Teller lattice instability. The theory and notion of phonon domains consistently explain the ubiquitous pre-martensitic anomalies as natural consequences of incomplete phonon softening. The phonon domains are characterised by broken dynamic symmetry of lattice vibrations and deform through internal phonon relaxation in response to stress (a particular case of Le Chatelier's principle), leading to previously unexplored new domain phenomenon. Experimental evidence of phonon domains is obtained by in situ three-dimensional phonon diffuse scattering and Bragg reflection using high-energy synchrotron X-ray single-crystal diffraction, which observes exotic domain phenomenon fundamentally different from usual ferroelastic domain switching phenomenon. In light of the theory and experimental evidence of phonon domains and their roles in pre-martensitic phenomena, currently existing alternative opinions on martensitic precursor phenomena are revisited.
Ultrafast electron-phonon coupling at the metal-dielectric interface
Yao, Qiaomu
The pump-probe technique is an ultrafast spectroscopy method of detecting the dynamics of energy carriers such as electrons, phonons, and holes with transient thermal reflectance measurement. A laser beam is divided into a pump beam and probe beam with different wavelength or polarization and time delay. According to the transient reflectance result, this method could be applied to investigate the interaction between electron-phonon and electron-electron coupling with a high temporal resolution on the order of 10 femtoseconds. Energy transfer of photo-excited electrons in a metal film to the dielectric substrate at the metal-dielectric interface is important for understanding the ultrafast heat transfer process across the two materials. Many researches have been conducted in finding this energy transfer process in different materials. In this thesis, by measuring the transient reflectance variation, the two-temperature model (TTM) is used to analyze the interface metal electron and dielectric substrate coupling. In order to relate temperature to the reflectance change, a temperature and wavelength dependent Drude-Lorentz model was developed which represents the temperature dependent dielectric constant and can be used to calculate reflectance variation. Ultrafast pump-and-probe interband transition measurements on Au-Si samples were carried out, where the probe photon energy was chosen to be close to the interband transition threshold (ITT) of gold to minimize the influence of non-equilibrium or non-thermalized electrons on the optical response, and to increase the signal to noise ratio for reflectance change. In the experiment, different pump fluences have been used to test the transient reflectance variation on Au-Si samples of different thicknesses. The pump wavelength is taken as 800 nm while the probe wavelength is taken as 490 nm. A thick gold of 1000 nm thickness has been used to determine the electron-phonon coupling strength represented by a constant G 0
Integrated phononic crystal resonators based on adiabatically-terminated phononic crystal waveguides
Dehghannasiri, Razi; Pourabolghasem, Reza; Eftekhar, Ali Asghar; Adibi, Ali
2016-12-01
In this letter, we demonstrate a new design for integrated phononic crystal (PnC) resonators based on confining acoustic waves in a heterogeneous waveguide-based PnC structure. In this architecture, a PnC waveguide that supports a single mode at the desired resonance frequencies is terminated by two waveguide sections with no propagating mode at those frequencies (i.e., have mode gap). The proposed PnC resonators are designed through combining the spatial-domain and the spatial-frequency domain (i.e., the k-domain) analysis to achieve a smooth mode envelope. This design approach can benefit both membrane-based and surface-acoustic-wave-based architectures by confining the mode spreading in k-domain that leads to improved electromechanical excitation/detection coupling and reduced loss through propagating bulk modes.
Rotational character change of the one-phonon and two-phonon $\\gamma$ vibration in odd-$A$ nuclei
Matsuzaki, Masayuki
2014-01-01
\\item[Background] The $\\gamma$ vibration is the most typical low-lying collective motion prevailing the nuclear chart. But only few one-phonon rotational bands in odd-$A$ nuclei have been known. Furthermore, two-phonon states, even the band head, have been observed in a very limited number of nuclides not only of odd-$A$ but even-even. \\item[Purpose] Among them, that in $^{105}$Mo is unique in that Coriolis effects are expected to be stronger than in $^{103}$Nb and $^{105}$Nb on which theoretical studies were reported. Then the purpose of the present work is to study $^{105}$Mo paying attention to rotational character change of the one-phonon and two-phonon bands in comparison with the present author's previous studies on $^{103}$Nb and $^{105}$Nb. \\item[Method] The particle-vibration coupling model based on the cranking model and the random-phase approximation is used to calculate the vibrational states in rotating odd-$A$ nuclei. \\item[Results] The present model reproduces the observed yrast zero-phonon and...
Reprint of : Absorbing/Emitting Phonons with one dimensional MOSFETs
Bosisio, Riccardo; Gorini, Cosimo; Fleury, Geneviève; Pichard, Jean-Louis
2016-08-01
We consider nanowires in the field effect transistor device configuration. Modeling each nanowire as a one dimensional lattice with random site potentials, we study the heat exchanges between the nanowire electrons and the substrate phonons, when electron transport is due to phonon-assisted hops between localized states. Shifting the nanowire conduction band with a metallic gate induces different behaviors. When the Fermi potential is located near the band center, a bias voltage gives rise to small local heat exchanges which fluctuate randomly along the nanowire. When it is located near one of the band edges, the bias voltage yields heat currents which flow mainly from the substrate towards the nanowire near one boundary of the nanowire, and in the opposite direction near the other boundary. This opens interesting perspectives for heat management at submicron scales: arrays of parallel gated nanowires could be used for a field control of phonon emission/absorption.
Temperature Dependent Variations of Phonon Interactions in Nanocrystalline Cerium Oxide
Directory of Open Access Journals (Sweden)
Sugandha Dogra Pandey
2015-01-01
Full Text Available The temperature dependent anharmonic behavior of the phonon modes of nanocrystalline CeO2 was investigated in the temperature range of 80–440 K. The anharmonic constants have been derived from the shift in phonon modes fitted to account for the anharmonic contributions as well as the thermal expansion contribution using the high pressure parameters derived from our own high pressure experimental data reported previously. The total anharmonicity has also been estimated from the true anharmonicity as well as quasiharmonic component. In the line-width variation analysis, the cubic anharmonic term was found to dominate the quartic term. Finally, the phonon lifetime also reflected the trend so observed.
Dynamics of Phononic Dissipation at the Atomic Scale
Sevincli, Haldun; Mukhopadhay, Soma; Tugrul Senger, R.; Ciraci, Salim
2007-03-01
Dynamics of dissipation of a local phonon distribution to the bulk is a key issue in boundary lubrication and friction between sliding surfaces. We consider a highly excited molecule which interacts weakly with the substrate surface. We study different types of coupling and substrates having different types of dimensionality and phonon densities of states. We propose three different methods to solve the dynamics of the combined system, namely the equation of mation technique, Fano-Anderson method and the Green's function method. Using this theoretical framework we present an analysis of transient properties of energy dissipation via phonon discharge at the microscopic level. The methods allow the theoretical calculations to be extended to include any density of states for the substrate including experimental ones and any type of molecule that represent the lubricant or the asperity.
Photonic-phononic orbital angular momentum in Brillouin parametric conversion
Zhu, Zhihan; Mu, Chunyuan; Li, Hongwei
2014-01-01
Orbital angular momentum (OAM) is a fundamental photonic degree of freedom, showed by Allen and co-workers. Its most attractive feature is an inherently infinite dimensionality, which in recent years has obtained several ground-breaking demonstrations for high information-density communication and processing, both in classical and quantum. Here, by seeking the reason for photonic OAM non-conservation in stimulated Brillouin amplification, we report the first demonstration of the evolution law for OAM in Brillouin process. The parameter of OAM can conveniently transfer between the phonons and different polarized photons due to the photonic spin angular momentum conservation. Our results have revealed a parametric conversion mechanism of Brillouin process for Photonic-phononic OAM, demonstrated the role of phononic OAM and the vortex acoustic wave in this process, and suggested this mechanism may find important applications in OAM-based information communication and processing.
Research Update: Phonon engineering of nanocrystalline silicon thermoelectrics
Directory of Open Access Journals (Sweden)
Junichiro Shiomi
2016-10-01
Full Text Available Nanocrystalline silicon thermoelectrics can be a solution to improve the cost-effectiveness of thermoelectric technology from both material and integration viewpoints. While their figure-of-merit is still developing, recent advances in theoretical/numerical calculations, property measurements, and structural synthesis/fabrication have opened up possibilities to develop the materials based on fundamental physics of phonon transport. Here, this is demonstrated by reviewing a series of works on nanocrystalline silicon materials using calculations of multiscale phonon transport, measurements of interfacial heat conduction, and synthesis from nanoparticles. Integration of these approaches allows us to engineer phonon transport to improve the thermoelectric performance by introducing local silicon-oxide structures.
Classification of topological phonons in linear mechanical metamaterials.
Süsstrunk, Roman; Huber, Sebastian D
2016-08-16
Topological phononic crystals, alike their electronic counterparts, are characterized by a bulk-edge correspondence where the interior of a material dictates the existence of stable surface or boundary modes. In the mechanical setup, such surface modes can be used for various applications such as wave guiding, vibration isolation, or the design of static properties such as stable floppy modes where parts of a system move freely. Here, we provide a classification scheme of topological phonons based on local symmetries. We import and adapt the classification of noninteracting electron systems and embed it into the mechanical setup. Moreover, we provide an extensive set of examples that illustrate our scheme and can be used to generate models in unexplored symmetry classes. Our work unifies the vast recent literature on topological phonons and paves the way to future applications of topological surface modes in mechanical metamaterials.
Classification of topological phonons in linear mechanical metamaterials
Süsstrunk, Roman; Huber, Sebastian D.
2016-08-01
Topological phononic crystals, alike their electronic counterparts, are characterized by a bulk-edge correspondence where the interior of a material dictates the existence of stable surface or boundary modes. In the mechanical setup, such surface modes can be used for various applications such as wave guiding, vibration isolation, or the design of static properties such as stable floppy modes where parts of a system move freely. Here, we provide a classification scheme of topological phonons based on local symmetries. We import and adapt the classification of noninteracting electron systems and embed it into the mechanical setup. Moreover, we provide an extensive set of examples that illustrate our scheme and can be used to generate models in unexplored symmetry classes. Our work unifies the vast recent literature on topological phonons and paves the way to future applications of topological surface modes in mechanical metamaterials.
Anomalous phonon behaviour in V sub 3 Si
Yethiraj, M
2002-01-01
In earlier studies of phonons in V sub 3 Si, a gradual softening of the (hh0) branch was observed and attributed to the martensitic transition in this compound, which precedes the onset of superconductivity by a few degrees K. In this work, the temperature dependence of the transverse acoustic (TA) branch along the hh0 direction was studied in greater detail and it is shown that while the TA hh0 mode starts to soften at relatively high temperatures (>200 K), an anomalous softening, which is rather localized in q, occurs just below T sub c. The intensity of this soft-phonon peak correlates extremely well with the onset of the superconducting phase and appears to vary as the order parameter with temperature and applied field. The similarities in the phonon softening and Fermi-surface anisotropy between this compound and the rare-earth nickel borocarbides suggest the existence of a common mechanism for the superconducting transition. (orig.)
Microwave-frequency electromechanical resonators incorporating phononic crystals
Satzinger, K. J.; Peairs, G.; Vainsencher, A.; Cleland, A. N.
Piezoelectric micromechanical resonators at gigahertz frequencies have been operated in the quantum limit, with quantum control and measurement achieved using superconducting qubits. However, experiments to date have been limited by mechanical dissipation, due to a combination of internal and radiative losses. In this talk, we explore the incorporation of phononic crystals into resonator designs. In phononic crystals, periodic patterning manipulates the acoustic band structure of the material. Through appropriately chosen geometries, these periodic patterns lead to full acoustic bandgaps which can be used to greatly reduce radiation losses from resonant structures. Alternatively, the crystal geometry can be manipulated to allow isolated modes within the bandgap, giving fine control over the spatial structure of the resonator modes. In this talk, we will describe the design, fabrication, and measurement of resonators with phononic crystals.
Electron-phonon coupling in perovskites studied by Raman Scattering
Sathe, V. G.; Tyagi, S.; Sharma, G.
2016-10-01
Raman scattering is an unique technique for characterization and quantification of electron-phonon, spin-phonon and spin-lattice coupling in many of the currently prominent compounds like multiferroics and manganites. In manganites, it is understood now that a phase separated landscape with coexisting metallic and insulating regions exist in most of the compounds and application of small external perturbation causes an alteration in this landscape. In such scenario, local metallic regions grow suddenly at the expense of insulating regions below the magnetic ordering temperature. Such regions can be characterized effectively using Raman scattering measurements where delocalized electrons couple with the adjacent phonon peaks giving a Fano resonance in the form of asymmetric line shape.
High temperature phonon dispersion in graphene using classical molecular dynamics
Energy Technology Data Exchange (ETDEWEB)
Anees, P., E-mail: anees@igcar.gov.in; Panigrahi, B. K. [Materials Physics Division, Indira Gandhi Centre for Atomic Research, Kalpakkam-603102 (India); Valsakumar, M. C., E-mail: anees@igcar.gov.in [School of Engineering Sciences and Technology, University of Hyderabad, Hyderabad-500046 (India)
2014-04-24
Phonon dispersion and phonon density of states of graphene are calculated using classical molecular dynamics simulations. In this method, the dynamical matrix is constructed based on linear response theory by computing the displacement of atoms during the simulations. The computed phonon dispersions show excellent agreement with experiments. The simulations are done in both NVT and NPT ensembles at 300 K and found that the LO/TO modes are getting hardened at the Γ point. The NPT ensemble simulations capture the anharmonicity of the crystal accurately and the hardening of LO/TO modes is more pronounced. We also found that at 300 K the C-C bond length reduces below the equilibrium value and the ZA bending mode frequency becomes imaginary close to Γ along K-Γ direction, which indicates instability of the flat 2D graphene sheets.
Electromagnetic excitation of phonons at C(001) surfaces
Energy Technology Data Exchange (ETDEWEB)
Perez-Sanchez, F L [Escuela de Ciencias, Universidad Autonoma ' Benito Juarez' de Oaxaca, Avenida Universidad S/N, Ex-Hacienda de Cinco Senores, Ciudad Universitaria, Oaxaca de Juarez, Oaxaca, 68120 (Mexico); Perez-Rodriguez, F, E-mail: fperez@sirio.ifuap.buap.m [Instituto de Fisica, Benemerita Universidad Autonoma de Puebla, Apartado Post. J-48, Puebla 72570 (Mexico)
2009-09-02
The photon-phonon coupling at C(001)-(2 x 1) surfaces and its manifestation in far-infrared reflectance anisotropy spectra (FIR-RAS) are theoretically investigated. We solve the coupled system of equations for the electromagnetic field and lattice vibrations, described within the adiabatic bond charge model (ABCM), with the method of expansion into bulk phonon and photon modes. The calculated FIR-RAS exhibit resonances associated with zone-center surface phonons in good agreement with available HREELS experiments and predictions of vibrational modes for diamond (001)-(2 x 1) surfaces from ABCM and ab initio calculations. Interestingly, the reflectance anisotropy spectra for a C(001)-(2 x 1) surface turn out to be qualitatively different from the spectra for a Si(001)-(2 x 1) surface, reported previously.
Li, Zi; Wang, Cong; Zhao, Jize; Kang, Wei; Zhang, Ping
2017-02-01
Rapid laser heating is an important experimental technique to achieve extreme conditions for uranium. Theoretical simulations of the electron-ion nonequilibrium energy relaxation after laser heating usually employ a two-temperature model using the thermal quantities of the electron heat capacity and the electron-phonon coupling factor as input parameters. Based on the first-principles calculations of the electron density of states and Eliashberg function, we theoretically determine the thermal quantities and their dependence on electron temperature and external pressure for uranium and revealed the connection between the thermal quantities and the electron density of states. The electron/ion temperature evolution was examined by employing the two-temperature model with the obtained thermal quantities. The time/temperature at the peak/equilibrium point of the temperature evolution curve was examined for different external pressures and different laser energy densities. We found that the approximation of a linear temperature-dependent electron heat capacity is acceptable at a low energy density, while at a high energy density, the electron temperature dependence of the electron heat capacity and the coupling factor from the first-principles calculations must be considered.
Unraveling the acoustic electron-phonon interaction in graphene
DEFF Research Database (Denmark)
Kaasbjerg, Kristen; Thygesen, Kristian S.; Jacobsen, Karsten W.
2012-01-01
Using a first-principles approach we calculate the electron-phonon couplings in graphene for the transverse and longitudinal acoustic phonons. Analytic forms of the coupling matrix elements valid in the long-wavelength limit are found to give an almost quantitative description of the first...... that the intrinsic effective acoustic deformation potential of graphene is Ξeff=6.8 eV and that the temperature dependence of the mobility μ~T-α in the Bloch-Gru¨neisen regime increases beyond an α=4 dependence even in the absence of screening when the true coupling matrix elements are considered. The α>4...
Electron-phonon interaction in high temperature superconductors
Directory of Open Access Journals (Sweden)
H. Khosroabadi
2006-09-01
Full Text Available We explore the important role of the strong electron-phonon interaction in high temperature superconductivity through the study of the results of some important experiments, such as inelastic neutron and X-ray scattering, angle resolved photoemission spectroscopy, and isotope effects. We also present our computational results of the eigenvalues and eigenvectors of the Ag Raman modes, and the ionic displacement dependence of the electronic band structure by density functional theory. It is clearly evident that the role of phonons in the mechanism behind the high-temperature superconducting state should be seriously considered.
The inverted pendulum, interface phonons and optic Tamm states
Combe, Nicolas
2011-01-01
The propagation of waves in periodic media is related to the parametric oscillators. We transpose the possibility that a parametric pendulum oscillates in the vicinity of its unstable equilibrium positions to the case of waves in lossless unidimensional periodic media. This concept formally applies to any kind of wave. We apply and develop it to the case of phonons in realizable structures and evidence new classes of phonons. Discussing the case of electromagnetic waves, we show that our concept is related to optic Tamm states one but extends it to periodic Optic Tamm state.
Coherent phonon coupling to individual Bloch states in photoexcited bismuth.
Papalazarou, E; Faure, J; Mauchain, J; Marsi, M; Taleb-Ibrahimi, A; Reshetnyak, I; van Roekeghem, A; Timrov, I; Vast, N; Arnaud, B; Perfetti, L
2012-06-22
We investigate the temporal evolution of the electronic states at the bismuth (111) surface by means of time- and angle-resolved photoelectron spectroscopy. The binding energy of bulklike bands oscillates with the frequency of the A(1g) phonon mode, whereas surface states are insensitive to the coherent displacement of the lattice. A strong dependence of the oscillation amplitude on the electronic wave vector is correctly reproduced by ab initio calculations of electron-phonon coupling. Besides these oscillations, all the electronic states also display a photoinduced shift towards higher binding energy whose dynamics follows the evolution of the electronic temperature.
Homogenization of Two-Dimensional Phononic Crystals at Low Frequencies
Institute of Scientific and Technical Information of China (English)
NI Qing; CHENG Jian-Chun
2005-01-01
@@ Effective velocities of elastic waves propagating in two-dimensional phononic crystal at low frequencies are analysed theoretically, and exact analytical formulas for effective velocities of elastic waves are derived according to the method presented by Krokhin et al. [Phys. Rev. Lett. 91 (2003) 264302]. Numerical calculations for phononic crystals consisted of array of Pb cylinders embedded in epoxy show that the composites have distinct anisotropy at low filling fraction. The anisotropy increases as the filling fraction increases, while as the filling fraction closes to the limitation, the anisotropy decreases.
Reconfigurable long-range phonon dynamics in optomechanical arrays
Xuereb, André; Pupillo, Guido; Paternostro, Mauro; Dantan, Aurélien
2013-01-01
We investigate periodic optomechanical arrays as reconfigurable platforms for engineering the coupling between multiple mechanical and electromagnetic modes and for exploring many-body phonon dynamics. Exploiting structural resonances in the coupling between light fields and collective motional modes of the array, we show that tunable effective long-range interactions between mechanical modes can be achieved. This paves the way towards the implementation of controlled phononic walks and heat transfer on densely-connected graphs as well as the coherent transfer of excitations between distant elements of optomechanical arrays.
Phonon Softening and Dispersion in EuTiO3
Ellis, David S.; UCHIYAMA, Hiroshi; Tsutsui, Satoshi; Sugimoto, Kunihisa; Kato, Kenichi; Ishikawa, Daisuke; Baron, Alfred Q. R.
2012-01-01
We measured phonon dispersion in single crystal EuTiO$_3$ using inelastic x-ray scattering. A structural transition to an antiferrodistortive phase was found at a critical temperature $T_0$=287$\\pm$1 K using powder and single-crystal x-ray diffraction. Clear softening of the zone boundary \\emph{R}-point \\textbf{q}=(0.5 0.5 0.5) acoustic phonon shows this to be a displacive transition. The mode energy plotted against reduced temperature could be seen to nearly overlap that of $\\rm SrTiO_3$, su...
Time Resolved Phonon Spectroscopy, Version 1.0
Energy Technology Data Exchange (ETDEWEB)
2016-12-22
TRPS code was developed for the project "Time Resolved Phonon Spectroscopy". Routines contained in this piece of software were specially created to model phonon generation and tracking within materials that interact with ionizing radiation, particularly applicable to the modeling of cryogenic radiation detectors for dark matter and neutrino research. These routines were created to link seamlessly with the open source Geant4 framework for the modeling of radiation transport in matter, with the explicit intent of open sourcing them for eventual integration into that code base.
Photons, phonons, and plasmons with orbital angular momentum in plasmas
Chen, Qiang; Liu, Jian
2016-01-01
Exact eigen modes with orbital angular momentum (OAM) in the complex media of unmagnetized homogeneous plasma are studied. Three exact eigen modes with OAM are discovered, i.e., photons, phonons, and plasmons. It is found that an OAM photon can be excited by two familiar Bessel modes without OAM. For the phonons and plasmons, their OAM are carried by the electrons and ions. The OAM modes in plasmas and their characteristics can be explored for various potential applications in plasma physics and accelerator physics.
Band structures and localization properties of aperiodic layered phononic crystals
Energy Technology Data Exchange (ETDEWEB)
Yan Zhizhong, E-mail: zzyan@bit.edu.cn [Department of Applied Mathematics, Beijing Institute of Technology, Beijing 100081 (China); Zhang Chuanzeng [Department of Civil Engineering, University of Siegen, D-57078 Siegen (Germany)
2012-03-15
The band structures and localization properties of in-plane elastic waves with coupling of longitudinal and transverse modes oblique propagating in aperiodic phononic crystals based on Thue-Morse and Rudin-Shapiro sequences are studied. Using transfer matrix method, the concept of the localization factor is introduced and the correctness is testified through the Rytov dispersion relation. For comparison, the perfect periodic structure and the quasi-periodic Fibonacci system are also considered. In addition, the influences of the random disorder, local resonance, translational and/or mirror symmetries on the band structures of the aperiodic phononic crystals are analyzed in this paper.
Band structures and localization properties of aperiodic layered phononic crystals
Yan, Zhi-Zhong; Zhang, Chuanzeng
2012-03-01
The band structures and localization properties of in-plane elastic waves with coupling of longitudinal and transverse modes oblique propagating in aperiodic phononic crystals based on Thue-Morse and Rudin-Shapiro sequences are studied. Using transfer matrix method, the concept of the localization factor is introduced and the correctness is testified through the Rytov dispersion relation. For comparison, the perfect periodic structure and the quasi-periodic Fibonacci system are also considered. In addition, the influences of the random disorder, local resonance, translational and/or mirror symmetries on the band structures of the aperiodic phononic crystals are analyzed in this paper.
Optical Conductivity of Graphene Sheet Including Electron-Phonon Interaction
Institute of Scientific and Technical Information of China (English)
Hamze Mousavi
2012-01-01
Using an expression of optical conductivity, based on the linear response theory, the Green＇s function technique and within the Holstein Hamiltonian model, the effect of electron-phonon interaction on the optical conductivity of graphene plane is studied. It is found that the electron-phonon coupling increases the optical conductivity of graphene sheet in the low frequency region due to decreasing quasiparticle weight of electron excitation while the optical conductivity reduces in the high frequency region. The latter is due to role of electrical field＇s frequency.
Flexural-Phonon Scattering Induced by Electrostatic Gating in Graphene
DEFF Research Database (Denmark)
Gunst, Tue; Kaasbjerg, Kristen; Brandbyge, Mads
2017-01-01
.We examine the effect of the gate-induced one-phonon scattering on the mobility for several gate geometries and dielectric environments using first-principles calculations based on density functional theory and the Boltzmann equation. We demonstrate that this scattering mechanism can be a mobility......-limiting factor, and show how the carrier density and temperature scaling of the mobility depends on the electrostatic environment. Our findings may explain the high deformation potential for in-plane acoustic phonons extracted from experiments and, furthermore, suggest a direct relation between device symmetry...
YPHON: A package for calculating phonons of polar materials
Wang, Yi; Chen, Long-Qing; Liu, Zi-Kui
2014-11-01
In our recent works, we have developed a mixed-space approach within the framework of direct method for the first-principle calculation of phonon properties. It makes full use of the accuracy of the force constants calculated in the real space and the dipole-dipole interactions in the reciprocal space, making the accurate phonon calculation possible with the direct method for polar materials. In this paper, an efficient C++ implementation of the mixed-space approach, YPHON, is provided as open source, including demos and Linux scripts for extracting input data to YPHON from the output of VASP.5. The functions of the current package include the calculations of: (1) the phonon dispersions; (2) the phonon density of states; (3) the neutron scattering section weighted phonon density of state; (4) the phonons of the high symmetry structure using the force constants from low symmetry structure; (5) the phonon dispersions of random alloys; and (6) the analysis of the vibrational modes using the point group theory. Catalogue identifier: AETS_v1_0 Program summary URL:http://cpc.cs.qub.ac.uk/summaries/AETS_v1_0.html Program obtainable from: CPC Program Library, Queen’s University, Belfast, N. Ireland Licensing provisions: Standard CPC licence, http://cpc.cs.qub.ac.uk/licence/licence.html No. of lines in distributed program, including test data, etc.: 567815 No. of bytes in distributed program, including test data, etc.: 9763594 Distribution format: tar.gz Programming language: C++, Linux scripts. Computer: Linux systems with a g++ or C++ compiler. Operating system: Linux. RAM: Ranges from a few Mbytes to a few Gbytes, dynamically depending on the system size. Classification: 7.8. External routines: GSL-the GNU Scientific Library (GSL) is a numerical library for C and C++ programmers. VASP.5 or later for the calculations of force constants and dielectric constants and Born effective charge for polar materials. Nature of problem: This package has the purpose of computing
Phonon thermal transport in metallic glasses below 100 K
Energy Technology Data Exchange (ETDEWEB)
Matey, James Regis
1978-01-01
Measurements of the phonon thermal conductivity of a variety of metallic glasses were made. In each case, the temperature dependence and magnitude of the phonon thermal conductivity of the glassy metal was very similar to that characteristic of nonmetallic glasses. Variation of sound velocity measurements were made on a glassy palladium silicon alloy and a qualitative similarity was found between its behavior and the behavior of nonmetallic glasses. These findings and results from other laboratories have led to the conclusion that the localized excitations responsible for the anomalous behavior of nonmetallic glasses are also present in the metallic glasses.
Evidences of evanescent Bloch waves in Phononic Crystals
Romero-García, V; Castiñeira-Ibáñez, S; Garcia-Raffi, L M
2010-01-01
We show both experimentally and theoretically the evanescent behaviour of modes in the Band Gap (BG) of finite Phononic Crystal (PC). Based on experimental and numerical data we obtain the imaginary part of the wave vector in good agreement with the complex band structures obtained by the Extended Plane Wave Expansion (EPWE). The calculated and measured acoustic field of a localized mode out of the point defect inside the PC presents also evanescent behaviour. The correct understanding of evanescent modes is fundamental for designing narrow filters and wave guides based on Phononic Crystals with defects.
Dynamical Cooper pairing in nonequilibrium electron-phonon systems
Knap, Michael; Babadi, Mehrtash; Refael, Gil; Martin, Ivar; Demler, Eugene
2016-12-01
We analyze Cooper pairing instabilities in strongly driven electron-phonon systems. The light-induced nonequilibrium state of phonons results in a simultaneous increase of the superconducting coupling constant and the electron scattering. We demonstrate that the competition between these effects leads to an enhanced superconducting transition temperature in a broad range of parameters. Our results may explain the observed transient enhancement of superconductivity in several classes of materials upon irradiation with high intensity pulses of terahertz light, and may pave new ways for engineering high-temperature light-induced superconducting states.
Photons, phonons, and plasmons with orbital angular momentum in plasmas
Chen, Qiang; Qin, Hong; Liu, Jian
2017-01-01
Exact eigen modes with orbital angular momentum (OAM) in the complex media of unmagnetized homogeneous plasmas are studied. Three exact eigen modes with OAM are derived, i.e., photons, phonons, and plasmons. The OAM of different plasma components are closely related to the charge polarities. For photons, the OAM of electrons and ions are of the same magnitude but opposite direction, and the total OAM is carried by the field. For the phonons and plasmons, their OAM are carried by the electrons and ions. The OAM modes in plasmas and their characteristics can be explored for potential applications in plasma physics and accelerator physics. PMID:28164998
Phonon dilatation, dressed vibrons and two-vibron bound states localization in an adsorbed nanowire
Pouthier, Vincent,
2006-01-01
A special attention is paid to characterize the two-vibron bound state dynamics of an anharmonic molecular nanostructure coupled with a set of optical phonons. It is shown that the vibron-phonon coupling is responsible for a new dressing mechanism. The vibrons are accompanied by virtual phonons which account for the scaling of each phonon coordinate and for the dilatation of the corresponding wave function. As a result, the dynamics of the dressed vibrons is governed by an effective Hamiltoni...
Temperature dependence of the Raman-active phonon frequencies in indium sulfide
Gasanly, N. M.; Özkan, H.; Aydinli, A.; Yilmaz, İ.
1999-03-01
The temperature dependence of the Raman-active mode frequencies in indium sulfide was measured in the range from 10 to 300 K. The analysis of the temperature dependence of the A g intralayer optical modes show that Raman frequency shift results from the change of harmonic frequency with volume expansion and anharmonic coupling to phonons of other branches. The pure-temperature contribution (phonon-phonon coupling) is due to three- and four-phonon processes.
Theoretical study of the transverse acoustic phonons of GaSb at high pressure
Indian Academy of Sciences (India)
S Shinde; M Talati; Prafulla K Jha; S P Sanyal
2004-08-01
We have investigated the phonon dispersion curves and one-phonon density of states up to the pressure of 8 GPa using a theoretical model, namely the rigid ion model. The transverse acoustic phonons as a function of pressure have been compared with the recently measured inelastic neutron scattering data which show a strong softening near the zone boundaries. The calculated one-phonon density of states show pronounced shift in the peak positions with the increase in pressure.
Smirnova, N A; Mizusaki, T; Van Isacker, P; Smirnova, Nadya A.; Pietralla, Norbert; Mizusaki, Takahiro; Isacker, Piet Van
2000-01-01
The interrelation between the octupole phonon and the low-lyingproton-neutron mixed-symmetry quadrupole phonon in near-spherical nuclei isinvestigated. The one-phonon states decay by collective E3 and E2 transitionsto the ground state and by relatively strong E1 and M1 transitions to theisoscalar 2^+ state. We apply the proton-neutron version of the InteractingBoson Model including quadrupole and octupole bosons (sdf-IBM-2). Two F-spinsymmetric dynamical symmetry limits of the model, namely the vibrational andthe $\\gamma$-unstable ones, are considered. We derive analytical formulae forexcitation energies as well as B(E1), B(M1), B(E2) and B(E3) values for anumber of transitions between low-lying states. The model well reproduces manyknown transition strengths in the near spherical nuclei ^{142}Ce and ^{94}Mo.
Directory of Open Access Journals (Sweden)
O.Yu. Guseva
2009-09-01
Full Text Available Biochemical changes in oral fluid of patients with chronic generalized parodontitis were investigated; the most informative indices were found out, they were used for estimating complex therapy effectiveness by means of low intensive helium — neon laser radiation and alternating running magnetic field
Khan, Mohammed Zahed Mustafa
2013-03-04
We report on the atypical emission dynamics of InAs/AlGaInAs/InP quantum dash (Qdash) lasers employing varying AlGaInAs barrier thickness (multilayer-chirped structure). The analysis is carried out via fabry-perot (FP) ridge (RW) and stripe waveguide (SW) laser characterization corresponding to the index and gain guided waveguiding mechanisms, respectively, and at different current pulse width operations. The laser emissions are found to emerge from the size dispersion of the Qdash ensembles across the four Qdash-barrier stacks, and governed by their overlapping quasi-zero dimensional density of states (DOS). The spectral characteristics demonstrated prominent dependence on the waveguiding mechanism at quasi-continuous wave (QCW) operation (long pulse width). The RW geometry showed unusual spectral split in the emission spectra on increasing current injection while the SW geometry showed typical broadening of lasing spectra. These effects were attributed to the highly inhomogeneous active region, the nonequilibrium carrier distribution and the energy exchange between Qdash groups across the Qdash-barrier stacks. Furthermore, QCW operation showed a progressive red shift of emission spectra with injection current, resulted from active region heating and carrier depopulation, which was observed to be minimal in the short pulse width (SPW) operation. Our investigation sheds light on the device physics of chirped Qdash laser structure and provides guidelines for further optimization in obtaining broad-gain laser diodes. © (2013) COPYRIGHT Society of Photo-Optical Instrumentation Engineers (SPIE). Downloading of the abstract is permitted for personal use only.
Two-phonon capture processes into quantum dots: The role of intermediate states
DEFF Research Database (Denmark)
Magnúsdóttir, Ingibjörg; Uskov, A. V.; Bischoff, Svend;
2003-01-01
We present a study of carrier capture into quantum dots via emission of longitudinal optical phonons. Two-phonon capture times are found to be of the order of some picoseconds at carrier densities 10^1^7cm^-^3 in situations where single-phonon capture processes are energetically prohibited. The i...
Relaxation between electrons and surface phonons of a homogeneously photoexcited metal film
Indian Academy of Sciences (India)
Navinder Singh
2004-11-01
The energy relaxation between the hot degenerate electrons of a homogeneously photoexcited metal film and the surface phonons (phonon wave vectors in two dimensions) is considered under Debye approximation. The state of electrons and phonons is described by equilibrium Fermi and Bose functions with different temperatures. Two cases for electron scattering by the metal surface, namely specular and diffuse scattering, are considered.
The Influence of Surface Phonons on Polaron States in Quantum Dots
Maslov, A. Yu.; Proshina, O. V.; Rusina, A. N.
2007-04-01
The influence of the surface phonons on the polaron effect in a quantum dot is investigated. We consider the polar quantum dot embedded into the polar matrix. The polaron energy shift for the electron and hole ground states is calculated. It is shown that the contribution of the surface phonons may exceed the bulk phonon contribution.
DEFF Research Database (Denmark)
Nielsen, Per Kær; Nielsen, Torben Roland; Lodahl, P.
2012-01-01
of the physics and emphasize the important role played by the effective phonon density, describing the availability of phonons for scattering, in quantum dot decay dynamics. Based on the analytical expressions, we present the parameter regimes where phonon effects are expected to be important. Also, we include...
Laser Processing and Chemistry
Bäuerle, Dieter
2011-01-01
This book gives an overview of the fundamentals and applications of laser-matter interactions, in particular with regard to laser material processing. Special attention is given to laser-induced physical and chemical processes at gas-solid, liquid-solid, and solid-solid interfaces. Starting with the background physics, the book proceeds to examine applications of lasers in “standard” laser machining and laser chemical processing (LCP), including the patterning, coating, and modification of material surfaces. This fourth edition has been enlarged to cover the rapid advances in the understanding of the dynamics of materials under the action of ultrashort laser pulses, and to include a number of new topics, in particular the increasing importance of lasers in various different fields of surface functionalizations and nanotechnology. In two additional chapters, recent developments in biotechnology, medicine, art conservation and restoration are summarized. Graduate students, physicists, chemists, engineers, a...
INTRODUCTION: Surface Dynamics, Phonons, Adsorbate Vibrations and Diffusion
Bruch, L. W.
2004-07-01
understanding of the underlying factors determining the optical quality of GaInNAs, such as composition, growth and annealing conditions. We are still far from establishing an understanding of the band structure and its dependence on composition. Fundamental electronic interactions such as electron-electron and electron-phonon scattering, dependence of effective mass on composition, strain and orientation, quantum confinement effects, effects of localized nitrogen states on high field transport and on galvanometric properties, and mechanisms for light emission in these materials, are yet to be fully understood. Nature and formation mechanisms of grown-in and processing-induced defects that are important for material quality and device performance are still unknown. Such knowledge is required in order to design strategies to efficiently control and eliminate harmful defects. For many potential applications (such as solar cells, HBTs) it is essential to get more information on the transport properties of dilute nitride materials. The mobility of minority carriers is known to be low in GaInNAs and related material. The experimental values are far from reaching the theoretical ones, due to defects and impurities introduced in the material during the growth. The role of the material inhomogeneities on the lateral carrier transport also needs further investigation. From the device's point of view most attention to date has been focused on the GaInNAs/GaAs system, mainly because of its potential for optoelectronic devices covering the 1.3-1.55 µm data and telecommunications wavelength bands. As is now widely appreciated, these GaAs-compatible structures allow monolithic integration of AlGaAs-based distributed Bragg reflector mirrors (DBRs) for vertical cavity surface-emitting lasers with low temperature sensitivity and compatibility with AlOx-based confinement techniques. In terms of conventional edge-emitting lasers (EELs), the next step is to extend the wavelength range for cw room
SQUEEZING PROPERTIES OF A TRAPPED ION IN THE STANDING-WAVE LASER
Institute of Scientific and Technical Information of China (English)
FANG MAO-FA; LIU XIANG
2001-01-01
We investigate the squeezing properties of a trapped ion in a standing-wave laser. Our results show that the squeezing of a trapped ion in the standing-wave laser is dependent on its position in the latter, the detuning parameter and the initial average phonon number.
Institute of Scientific and Technical Information of China (English)
ZHANGLi; Hong-Jing; CHENChuan-Yu
2003-01-01
By using determinant method as in our recent work, the IO phonon modes, the orthogonal relation for polarization vector, electron-IO phonon F~6hlich interaction Hamiltonian, the dispersion relation, and the electron-phonon coupling function in an arbitrary layer-number quantum well system have been derived and investigated within the framework of dielectric continuum approximation. Numerical calculation on seven-layer AlxGal-xAs/GaAs systems have been performed. Via the numerical results in this work and previous works, the general characters of the IO phonon modes in an n-layer coupling quantum well system were concluded and summarized. This work can be regarded as a generalization of previous works on IO phonon modes in some fLxed layer-number quantum well systems, and it provides a uniform method to investittate the effects of IO phonons on the multi-layer coupling quantum well systems.
Phonon and thermal properties of achiral single wall carbon nanotubes
Indian Academy of Sciences (India)
Prapti Saxena; Sankar P Sanyal
2006-08-01
A detailed theoretical study of the phonon and thermal properties of achiral single wall carbon nanotubes has been carried out using force constant model considering up to third nearest-neighbor interactions. We have calculated the phonon dispersions, density of states, radial breathing modes (RBM) and the specific heats for various zigzag and armchair nanotubes, with radii ranging from 2.8 Å to 11.0 Å. A comparative study of phonon spectrum with measured Raman data reveals that the number of Raman active modes for a tube does not depend on the number of atoms present in the unit cell but on its chirality. Calculated phonon modes at the zone center more or less accurately predicted the Raman active modes. The radial breathing mode is of particular interest as for a specific radius of a nanotube it is found to be independent of its chirality. We have also calculated the variation of RBM and G-band modes for tubes of different radii. RBM shows an inverse dependence on the radius of the tube. Finally, the values of specific heat are calculated for various nanotubes at room temperature and it was found that the specific heat shows an exponential dependence on the diameter of the tube.
Phonon transport in single-layer boron nanoribbons
Zhang, Zhongwei; Xie, Yuee; Peng, Qing; Chen, Yuanping
2016-11-01
Inspired by the successful synthesis of three two-dimensional (2D) allotropes, the boron sheet has recently been one of the hottest 2D materials around. However, to date, phonon transport properties of these new materials are still unknown. By using the non-equilibrium Green’s function (NEGF) combined with the first principles method, we study ballistic phonon transport in three types of boron sheets; two of them correspond to the structures reported in the experiments, while the third one is a stable structure that has not been synthesized yet. At room temperature, the highest thermal conductance of the boron nanoribbons is comparable with that of graphene, while the lowest thermal conductance is less than half of graphene’s. Compared with graphene, the three boron sheets exhibit diverse anisotropic transport characteristics. With an analysis of phonon dispersion, bonding charge density, and simplified models of atomic chains, the mechanisms of the diverse phonon properties are discussed. Moreover, we find that many hybrid patterns based on the boron allotropes can be constructed naturally without doping, adsorption, and defects. This provides abundant nanostructures for thermal management and thermoelectric applications.
Phonons in A3C60 Lattice and Structural Dynamics
Directory of Open Access Journals (Sweden)
Sven Larsson
2010-01-01
Full Text Available The critical temperature ( of superconductivity in A3C60 compounds is generally lower smaller with alkali atoms (A. Furthermore decreases with applied pressure. In the BCS model, these trends are explained by the lower density of states at the Fermi level for a decreased lattice constant (R. There is more than one counterexample, however, suggesting that BCS does not give the whole truth. The most important one is that the compound with the largest lattice constant, Cs3C60, is not superconducting at all at ambient pressure. In this paper we derive a novel model where a negative lattice contribution to Hubbard U, proportional to 1/R, is taken into account. It is possible to explain why A3C60 compounds with A = Li, and Na have a low or are not superconducting at all, and why Cs3C60 is superconducting only at applied pressure and then with the highest of all C60 alkali fullerides. It is concluded that the density of states mechanism derived in the BCS model is in doubt. Nevertheless superconductivity in A3C60 depends on electron-phonon coupling. The dominating phonon is the bond stretching Ag phonon, a breathing phonon for the whole fullerene molecular ion.
Electron-phonon coupling using many-body GW theory
Monserrat, Bartomeu; Vanderbilt, David
Electron-phonon coupling drives a plethora of phenomena, such as superconductivity in metals, or the temperature dependence of optical properties in semiconductors. There is increasing evidence that semi-local density functional theory (DFT) is not adequate for the description of electron-phonon coupling, and instead effects such as electronic correlation need to be included. Unfortunately, methods beyond semi-local DFT are computationally demanding, limiting the study of these phenomena. In this talk we will introduce the idea of ``thermal lines'', which can be used to explore the vibrational phase space of solids and molecules at small computational cost. In particular, we will describe how thermal lines can be exploited to calculate the temperature dependence of band structures beyond semi-local DFT, by using many-body GW theory, or by including the effects of spin-orbit coupling. We will present first-principles results showing the effects of electron correlation on the strength of electron-phonon coupling, and the effects of electron-phonon coupling on topological states of matter. Supported by Robinson College, Cambridge, and the Cambridge Philosophical Society.
Long-Wavelength Phonon Scattering in Nonpolar Semiconductors
DEFF Research Database (Denmark)
Lawætz, Peter
1969-01-01
The long-wavelength acoustic- and optical-phonon scattering of carriers in nonpolar semiconductors is considered from a general point of view. The deformation-potential approximation is defined and it is shown that long-range electrostatic forces give a nontrivial correction to the scattering. Fo...
Toward Single Electron Resolution Phonon Mediated Ionization Detectors
Mirabolfathi, Nader; Mahapatra, Rupak; Sundqvist, Kyle; Jastram, Andrew; Serfass, Bruno; Faiez, Dana; Sadoulet, Bernard
2015-01-01
Experiments seeking to detect rare event interactions such as dark matter or coherent elastic neutrino nucleus scattering are striving for large mass detectors with very low detection threshold. Using Neganov-Luke phonon amplification effect, the Cryogenic Dark Matter Search (CDMS) experiment is reaching unprecedented RMS resolutions of ~ 14 eV$_{ee}$ . CDMSlite is currently the most sensitive experiment to WIMPs of mass $\\sim$5 GeV/c$^{2}$ but is limited in achieving higher phonon gains due to an early onset of leakage current into Ge crystals. The contact interface geometry is particularly weak for blocking hole injection from the metal, and thus a new design is demonstrated that allows high voltage bias via vacuum separated electrode. With an increased bias voltage and a $\\times$ 2 Luke phonon gain, world best RMS resolution of sigma $\\sim$7 eV$_{ee}$ for 0.25 kg (d=75 mm, h=1 cm) Ge detectors was achieved. Since the leakage current is a function of the field and the phonon gain is a function of the applie...
Coalescence towards exceptional contours in synthetic phononic media
DEFF Research Database (Denmark)
Christensen, Johan
2016-01-01
are induced via the acousto-electric effect in electrically biased piezoelectric semiconductors. We study how wave attenuation and amplification can be tuned, and when combined, can give rise to phononic synthetic media with unidirectional suppressed reflectance, a feature directly applicable to evading sonar...
WAVE PROPAGATION IN TWO-DIMENSIONAL DISORDERED PIEZOELECTRIC PHONONIC CRYSTALS
Institute of Scientific and Technical Information of China (English)
Jinqiang Li; Fengming Li; Yuesheng Wang; Kikuo Kishimoto
2008-01-01
The wave propagation is studied in two-dimensional disordered piezoelectric phononie crystals using the finite-difference time-domain (FDTD) method. For different eases of disorder,the transmission coefficients are calculated. The influences of disorders on band gaps are investigated. The results show that the disorder in the piezoelectric phononic crystals has more significant influences on the band gap in the low frequency regions than in the high frequency ones. The relation between the width of band gap and the direction of position disorder is also discussed. When the position disorder is along the direction perpendicular to the wave transmission, the piezoelectric phononic crystals have wider band gaps at low frequency regions than the case of position disorder being along the wave transmission direction. It can also be found that the effect of. size disorder on band gaps is analogous to that of location disorder. When the perturbation coefficient is big, it has more pronounced effects on the pass bands in the piezoelectric phononic crystals with both size and location disorders than in the piezoelectric phononic crystals with single disorder.In higher frequency regions the piezoelectric effect reduces the transmission coefficients. But for larger disorder degree, the effects of the piezoelectricity will be reduced.
Quantum symmetries induced by phonons in the Hubbard model
Energy Technology Data Exchange (ETDEWEB)
Montorsi, A.; Rasetti, M. (Theory Division, Los Alamos National Laboratories, Los Alamos, New Mexico 87545 (United States) Dipartimento di Fisica and Unita Istituto Nazionale di Fisica della Materia, Politecnico di Torino, I-10129 Torino (Italy))
1994-03-14
We show how the addition of a phonon field to the Hubbard model deforms the [ital superconducting] su(2) part of the global symmetry Lie algebra su(2)[direct product]su(2)/[ital openZ][sub 2], holding at half filling for the customary model, into a [ital quantum] [su(2)][sub [ital q
Frictional drag between quantum wells mediated by phonon exchange
DEFF Research Database (Denmark)
Bønsager, M.C.; Flensberg, Karsten; Hu, Ben Yu-Kuang;
1998-01-01
lattice imperfections or electronic excitations is accounted for. In the case of GaAs quantum wells, we find that for a phonon mean free path l(ph) smaller than a critical value, imperfection scattering dominates and the drag rate varies as ln(l(ph)/d) over many orders of magnitude of the layer separation...
Enhanced Electron-Phonon Coupling at Metal Surfaces
Energy Technology Data Exchange (ETDEWEB)
Plummer, Ward E.
2010-08-04
The Born-Oppenheimer approximation (BOA) decouples electronic from nuclear motion, providing a focal point for most quantum mechanics textbooks. However, a multitude of important chemical, physical and biological phenomena are driven by violations of this approximation. Vibronic interactions are a necessary ingredient in any process that makes or breaks a covalent bond, for example, conventional catalysis or enzymatically delivered biological reactions. Metastable phenomena associated with defects and dopants in semiconductors, oxides, and glasses entail violation of the BOA. Charge exchange in inorganic polymers, organic slats and biological systems involves charge- induced distortions of the local structure. A classic example is conventional superconductivity, which is driven by the electron-lattice interaction. High-resolution angle-resolved photoemission experiments are yielding new insight into the microscopic origin of electron-phonon coupling (EPC) in anisotropic two-dimensional systems. Our recent surface phonon measurement on the surface of a high-Tc material clearly indicates an important momentum dependent EPC in these materials. In the last few years we have shifted our research focus from solely looking at electron phonon coupling to examining the structure/functionality relationship at the surface of complex transition metal compounds. The investigation on electron phonon coupling has allowed us to move to systems where there is coupling between the lattice, the electrons and the spin.
Hyperbolic phonon polaritons in hexagonal boron nitride (Conference Presentation)
Dai, Siyuan; Ma, Qiong; Fei, Zhe; Liu, Mengkun; Goldflam, Michael D.; Andersen, Trond; Garnett, William; Regan, Will; Wagner, Martin; McLeod, Alexander S.; Rodin, Alexandr; Zhu, Shou-En; Watanabe, Kenji; Taniguchi, T.; Dominguez, Gerado; Thiemens, Mark; Castro Neto, Antonio H.; Janssen, Guido C. A. M.; Zettl, Alex; Keilmann, Fritz; Jarillo-Herrero, Pablo; Fogler, Michael M.; Basov, Dmitri N.
2016-09-01
Uniaxial materials whose axial and tangential permittivities have opposite signs are referred to as indefinite or hyperbolic media. While hyperbolic responses are normally achieved with metamaterials, hexagonal boron nitride (hBN) naturally possesses this property due to the anisotropic phonons in the mid-infrared. Using scattering-type scanning near-field optical microscopy, we studied polaritonic phenomena in hBN. We performed infrared nano-imaging of highly confined and low-loss hyperbolic phonon polaritons in hBN. The polariton wavelength was shown to be governed by the hBN thickness according to a linear law persisting down to few atomic layers [1]. Additionally, we carried out the modification of hyperbolic response in meta-structures comprised of a mononlayer graphene deposited on hBN [2]. Electrostatic gating of the top graphene layer allows for the modification of wavelength and intensity of hyperbolic phonon polaritons in bulk hBN. The physics of the modification originates from the plasmon-phonon coupling in the hyperbolic medium. Furthermore, we demonstrated the "hyperlens" for subdiffractional focusing and imaging using a slab of hBN [3]. References [1] S. Dai et al., Science, 343, 1125 (2014). [2] S. Dai et al., Nature Nanotechnology, 10, 682 (2015). [3] S. Dai et al., Nature Communications, 6, 6963 (2015).
Phonon spectral densities of Cu surfaces: Application to Cu(211)
Mărinică, M.-C.; Raşeev, G.; Smirnov, K. S.
2001-05-01
Power phonon spectra of vicinal stepped surfaces of Cu(211) have been calculated using a molecular dynamics method combined with a semiempirical potential. The potential is based on an analytic form of inverse powers proposed by Finnis and Sinclair with the parametrization of Sutton and Chen. One of the four independent parameters of the potential was rescaled to reproduce the bulk phonon spectrum of Cu while retaining other properties of the bulk Cu close to the experimental values. Using this potential, we calculated the power surface phonon spectra, projection of the spectra at the high-symmetry points of surface Brillouin zone (SBZ), and the mean square displacements (MSD's) of atoms of the Cu(211) surface. The calculated projected phonon spectra at Γ¯ and at two new SBZ points (at X¯ and Y¯) compare favorably with experiment and theory when available. The MSD of the Cu(211) surface is also well reproduced and its temperature dependence shows that anharmonicity of the atomic motion becomes important above 200 K.
Energy Technology Data Exchange (ETDEWEB)
Rezende, Sandra Bastos
2001-07-01
In this research, it was analyzed the acceleration of the healing process of cutaneous lesions in mice, using a diode laser emitting in 830 nm. The 64 selected animals in this study were randomically divided into four groups of 16 animals each (G1, G2, G3 and G4). Biometric and histological comparisons were accomplished in the following periods: 3, 7 and 14 days after the surgery and laser application. Three laser irradiation configurations were used: a punctual contact (G2) and two non-contact and uniform (G3 and G4). For group G2, the laser intensity was 428 mW/cm{sup 2} , and for groups G3 and G4 it was 53 mW/cm{sup 2}. The total doses were D = 3 J/cm{sup 2} for groups G2 and G4, and D = 1,3 J/cm{sup 2} for G3. The first group, G1, was considered control and thus not submitted to any treatment after the surgery. All irradiated lesions presented acceleration of the healing process with regard to the control group. However, our results clearly indicate that the smaller laser intensity (uniform irradiation) leaded to the best results. On the other hand, the smaller used dose also leaded to the more significant and expressive results. The combination of the intensity value of 53 mW/cm{sup 2} and the dose of 1,3 J/cm{sup 2} leaded to optimal results, regarding the Biometric and histological analysis, presenting faster lesion contraction, quicker neoformation of epithelial and conjunctive tissue (with more collagen fibers ). (author)
Energy Technology Data Exchange (ETDEWEB)
Rocha, Dalva Maria
2001-07-01
This work was achieved in vivo and in vitro to evaluate the efficiency of Er:YAG laser in the cervical dentinal hypersensitivity treatment (HSDC). The Clinical study was achieved in patients with HSDC. The treatment was realized in five sessions: the first for selection, the second for exams (clinic and X-Ray) and trying to remove the etiologic factors that could cause the HSDC. The third and fourth sessions were subjected to the radiation with that protocol: 60 mJ energy ,2 Hz frequency, 6 mm out of focus, under air cooling, 20 seconds each application which the same was repeated four times with one minute breaks, which scanning movements and without using anaesthetics. The fifth was evaluation. The patients were evaluated and registered in a subject scale of pain 0 to 3, in the beginning and end of each session of irradiation, and one month after the last session. The results showed that for the irradiated group occurs significant differences in the beginning of each session and between. For the control group did not occur significant differences in the beginning and after each session, but did show a difference between the sessions. As the control group as the irradiated group, had reduction of sensibility between the session. For the morphologic study nine teeth were selected, 7 molars and 2 pre-molars from operative dentistry discipline. Half of the surface was irradiated with Er:YAG laser, the same protocol used in vivo, and the other half was used as a control without receiving any laser irradiation. Subsequently, specimens were prepared for SEM examinations. The results showed that laser treated surfaces showed a reduction of dentine tubular diameter with partial or total closure of the dentine tubules. For the control group, it was observed bigger amounts smear layer and open dentine tubular. The results obtained indicated that the Er:YAG laser can contribute to the HSDC treatment. (author)
Action semantics modulate action prediction.
Springer, Anne; Prinz, Wolfgang
2010-11-01
Previous studies have demonstrated that action prediction involves an internal action simulation that runs time-locked to the real action. The present study replicates and extends these findings by indicating a real-time simulation process (Graf et al., 2007), which can be differentiated from a similarity-based evaluation of internal action representations. Moreover, results showed that action semantics modulate action prediction accuracy. The semantic effect was specified by the processing of action verbs and concrete nouns (Experiment 1) and, more specifically, by the dynamics described by action verbs (Experiment 2) and the speed described by the verbs (e.g., "to catch" vs. "to grasp" vs. "to stretch"; Experiment 3). These results propose a linkage between action simulation and action semantics as two yet unrelated domains, a view that coincides with a recent notion of a close link between motor processes and the understanding of action language.
Optimal design of tunable phononic bandgap plates under equibiaxial stretch
Hedayatrasa, Saeid; Abhary, Kazem; Uddin, M. S.; Guest, James K.
2016-05-01
Design and application of phononic crystal (PhCr) acoustic metamaterials has been a topic with tremendous growth of interest in the last decade due to their promising capabilities to manipulate acoustic and elastodynamic waves. Phononic controllability of waves through a particular PhCr is limited only to the spectrums located within its fixed bandgap frequency. Hence the ability to tune a PhCr is desired to add functionality over its variable bandgap frequency or for switchability. Deformation induced bandgap tunability of elastomeric PhCr solids and plates with prescribed topology have been studied by other researchers. Principally the internal stress state and distorted geometry of a deformed phononic crystal plate (PhP) changes its effective stiffness and leads to deformation induced tunability of resultant modal band structure. Thus the microstructural topology of a PhP can be altered so that specific tunability features are met through prescribed deformation. In the present study novel tunable PhPs of this kind with optimized bandgap efficiency-tunability of guided waves are computationally explored and evaluated. Low loss transmission of guided waves throughout thin walled structures makes them ideal for fabrication of low loss ultrasound devices and structural health monitoring purposes. Various tunability targets are defined to enhance or degrade complete bandgaps of plate waves through macroscopic tensile deformation. Elastomeric hyperelastic material is considered which enables recoverable micromechanical deformation under tuning finite stretch. Phononic tunability through stable deformation of phononic lattice is specifically required and so any topology showing buckling instability under assumed deformation is disregarded. Nondominated sorting genetic algorithm (GA) NSGA-II is adopted for evolutionary multiobjective topology optimization of hypothesized tunable PhP with square symmetric unit-cell and relevant topologies are analyzed through finite
Probing and tuning inelastic phonon conductance across finite-thickness interface
Murakami, Takuru; Shiga, Takuma; Shiomi, Junichiro
2015-01-01
Phonon transmission across an interface between dissimilar crystalline solids is calculated using molecular dynamics simulations with interatomic force constants obtained from first principles. The results reveal that although inelastic phonon-transmission right at the geometrical interface can become far greater than the elastic one, its contribution to thermal boundary conductance (TBC) is severely limited by the transition regions, where local phonon states at the interface recover the bulk state over a finite thickness. This suggests TBC can be increased by enhancing phonon equilibration in the transition region for instance by phonon scattering, which is demonstrated by increasing the lattice anharmonicity.
Anti-Correlation between Energy-Gap and Phonon Energy for Cuprate Bi2212 Superconductor
Institute of Scientific and Technical Information of China (English)
FAN Wei
2008-01-01
Using the electron-phonon mechanism, we explain the spatial anti-correlation between the energy-gap and the energy of phonon mode for cuprate superconductor found in tunnelling spectrum by STM measurements of Bi2212, which is the direct effect of an important relationship (or constraint) I =const, where I is superconducting parameters. By relaxing above constraint, we study the correlation of energy gap and phonon energy when I has a distribution. We calculate a map of transition temperature in space constructing by phonon energy and the parameter of electron-phonon interaction, which is helpful for understanding of the relation.
Energy Technology Data Exchange (ETDEWEB)
Walverde, Debora Ayala
2001-07-01
This in vitro study compares two different types of tooth bleaching agents stimulated with two different irradiation fonts. These fonts accelerate the action of the bleaching agents upon the enamel surface by heating up the materials. We used the xenon plasma arc lamp and a 960 nm fiber-coupled diode laser to irradiate the two materials containing 35% of hydrogen peroxide (Opus White and Opalescence extra). The color of the teeth was measured with a spectrophotometer using the CIELAB color system that gives the numeric values of L{sup *}a{sup *}b{sup *}. (author)
Kosevich, Yury; Han, Haoxue; Volz, Sebastian
2014-03-01
We study theoretically phonon transmission through the interface between two solid crystals, which contains heavy isotopic impurities and/or soft-force-constant defects. We perform analytical calculations of plane wave transmission and numerical molecular dynamics simulation of wave packet transmission, which give consistent with each other results. If the impurities do not fill completely the interface plane, longitudinal and transverse phonons have two passes to cross such interface, through the host and through the impurity atoms bonds. Destructive interference between these passes can result in total resonance reflection of the phonon. The phonon transmission antiresonance is followed by phonon reflection antiresonance at higher frequency. The random distribution of the defects at the interface and nonlinearity of atomic bonds do not deteriorate the reflection and transmission antiresonances. Such Fano-like phonon interference antiresonances can affect heat transport through interfaces and contacts between nanostructures with impurities. The antiresonances are realized in phonon transmission through a planar defect in Si crystal with segregated Ge atoms. The phonon antiresonances can be considered as interference phenomena in atomic-scale phononic metamaterials.
Study of LO-phonon decay in semiconductors for hot carrier solar cell
Levard, Hugo; Vidal, Julien; Laribi, Sana; Guillemoles, Jean-François
2014-03-01
Knowledge of phonon decay is of crucial importance when studying basic properties of semiconductors, since they are closely related to Raman linewidth and non-equilibrium-hot-carriers cooling. The latter indeed cools down to the bottom of the conduction band within a picosecond range because of electron-phonon interaction. The eventual emitted hot phonons then decay in few picoseconds. The hot carriers cooling can be slowed down by considering the decay rate dependence of phonon on conservation rules, whose tuning may reduce the allowed two-phonon final states density. This is of direct interest for the third generation photovoltaic devices that are Hot Carrier Solar Cells (HCSC), in which the photoexcited carriers are extracted at an energy higher than thermal equilibrium. One of the HCSC main challenges then is to find an absorber material in which the hot phonons has a relaxation time longer than the carriers cooling time, so that we can expect the electron to ``reabsorb'' a phonon, slowing down the electronic cooling. HCSC yield is ultimately limited by LO phonon decay, though. In this work, we present theoretical results obtained from ab initio calculations of phonon lifetime in III-V and IV-IV semiconductors through a three-phonon process. Common approximations in the literature are questioned. In particular, we show that the usual ``zone-center approximation'' is not valid in some specific semiconductors. The analysis allows to correctly investigate phonon decay mechanisms in bulk and nanostructured materials.
Phonovoltaic. I. Harvesting hot optical phonons in a nanoscale p -n junction
Melnick, Corey; Kaviany, Massoud
2016-03-01
The phonovoltaic (pV) cell is similar to the photovoltaic. It harvests nonequilibrium (hot) optical phonons (Ep ,O) more energetic than the band gap (Δ Ee ,g) to generate power in a p-n junction. We examine the theoretical electron-phonon and phonon-phonon scattering rates, the Boltzmann transport of electrons, and the diode equation and hydrodynamic simulations to describe the operation of a pV cell and develop an analytic model predicting its efficiency. Our findings indicate that a pV material with Ep ,O≃Δ Ee ,g≫kBT , where kBT is the thermal energy, and a strong interband electron-phonon coupling surpasses the thermoelectric limit, provided the optical phonon population is excited in a nanoscale cell, enabling the ensuing local nonequilibrium. Finding and tuning a material with these properties is challenging. In Paper II [C. Melnick and M. Kaviany, Phys. Rev. B 93, 125203 (2016), 10.1103/PhysRevB.93.125203], we tune the band gap of graphite within density functional theory through hydrogenation and the application of isotropic strains. The band gap is tuned to resonate with its energetic optical phonon modes and calculate the ab initio electron-phonon and phonon-phonon scattering rates. While hydrogenation degrades the strong electron-phonon coupling in graphene such that the figure of merit vanishes, we outline the methodology for a continued material search.
Optical phonon lasing and its detection in transport through semiconduc- tor double quantum dots
Okuyama, Rin; Eto, Mikio; Brandes, Tobias
2014-03-01
We theoretically propose optical phonon lasing for a double quantum dot (DQD) fabricated in a semiconductor substrate. No additional cavity or resonator is required. We show that the DQD couples to only two phonon modes that act as a natural cavity. The pumping to the upper level is realized by an electric current through the DQD under a finite bias. Using the rate equation in the Born-Markov-Secular approximation, we analyze the enhanced phonon emission when the level spacing in the DQD is tuned to the phonon energy. We find the phonon lasing when the pumping rate is much larger than the phonon decay rate, whereas anti-bunching of phonon emission is observed when the pumping rate is smaller.[1] Our theory can be also applicable to DQDs embedded in nanomechanical resonators to control the vibrating modes. We discuss detection of amplified modes using the electric current and its noise through the DQD, and another DQD fabricated nearby.
Nomura, Yusuke; Arita, Ryotaro
2015-12-01
We formulate an ab initio downfolding scheme for electron-phonon-coupled systems. In this scheme, we calculate partially renormalized phonon frequencies and electron-phonon coupling, which include the screening effects of high-energy electrons, to construct a realistic Hamiltonian consisting of low-energy electron and phonon degrees of freedom. We show that our scheme can be implemented by slightly modifying the density functional-perturbation theory (DFPT), which is one of the standard methods for calculating phonon properties from first principles. Our scheme, which we call the constrained DFPT, can be applied to various phonon-related problems, such as superconductivity, electron and thermal transport, thermoelectricity, piezoelectricity, dielectricity, and multiferroicity. We believe that the constrained DFPT provides a firm basis for the understanding of the role of phonons in strongly correlated materials. Here, we apply the scheme to fullerene superconductors and discuss how the realistic low-energy Hamiltonian is constructed.
Femtosecond spectroscopy of electron-electron and electron-phonon energy relaxation in Ag and Au
Groeneveld, Rogier H. M.; Sprik, Rudolf; Lagendijk, Ad
1995-05-01
We show experimentally that the electron distribution of a laser-heated metal is a nonthermal distribution on the time scale of the electron-phonon (e-ph) energy relaxation time τE. We measured τE in 45-nm Ag and 30-nm Au thin films as a function of lattice temperature (Ti=10-300 K) and laser-energy density (Ul=0.3-1.3 J cm-3), combining femtosecond optical transient-reflection techniques with the surface-plasmon polariton resonance. The experimental effective e-ph energy relaxation time decreased from 710-530 fs and 830-530 fs for Ag and Au, respectively, when temperature is lowered from 300 to 10 K. At various temperatures we varied Ul between 0.3-1.3 J cm-3 and observed that τE is independent from Ul within the given range. The results were first compared to theoretical predictions of the two-temperature model (TTM). The TTM is the generally accepted model for e-ph energy relaxation and is based on the assumption that electrons and lattice can be described by two different time-dependent temperatures Te and Ti, implying that the two subsystems each have a thermal distribution. The TTM predicts a quasiproportional relation between τE and Ti in the perturbative regime where τE is not affected by Ul. Hence, it is shown that the measured dependencies of τE on lattice temperature and energy density are incompatible with the TTM. It is proven that the TTM assumption of a thermal electron distribution does not hold especially under our experimental conditions of low laser power and lattice temperature. The electron distribution is a nonthermal distribution on the picosecond time scale of e-ph energy relaxation. We developed a new model, the nonthermal electron model (NEM), in which we account for the (finite) electron-electron (e-e) and electron-phonon dynamics simultaneously. It is demonstrated that incomplete electron thermalization yields a slower e-ph energy relaxation in comparison to the thermalized limit. With the NEM we are able to give a consistent
Directory of Open Access Journals (Sweden)
Takashi Yatsui
2015-01-01
Full Text Available We compared dressed-photon-phonon (DPP etching to conventional photochemical etching and, using a numerical analysis of topographic images of the resultant etched polymethyl methacrylate (PMMA substrate, we determined that the DPP etching resulted in the selective etching of smaller scale structures in comparison with the conventional photochemical etching. We investigated the wavelength dependence of the PMMA substrate etching using an O2 gas. As the dissociation energy of O2 is 5.12 eV, we applied a continuous-wave (CW He-Cd laser (λ= 325 nm, 3.81 eV for the DPP etching and a 5th-harmonic Nd:YAG laser (λ= 213 nm, 5.82 eV for the conventional photochemical etching. From the obtained atomic force microscope images, we confirmed a reduction in surface roughness, Ra, in both cases. However, based on calculations involving the standard deviation of the height difference function, we confirmed that the conventional photochemical etching method etched the larger scale structures only, while the DPP etching process selectively etched the smaller scale features.
Directory of Open Access Journals (Sweden)
Aristides Palhares
2009-02-01
Full Text Available PURPOSE: To evaluate the effect of low intensity laser on the pseudocapsula contraction that occurs around silicone implants. METHODS: 60 male rats divided in two experimental groups received a silicone implant in the subcutaneous of the dorsal region. Group I: animals received implants in the subcutaneous dorsal region and did not receive any treatment; Group II: animals received seven irradiation sessions with low intensity laser after they had received subcutaneous implants. Thirty, 60 and 180 days after the surgery, tonometric evaluation of the implants was conducted. After that, the animals were sacrificed, study material was removed and prepared for histological examination. The thickness of the pseudocapsule and the inflammatory reaction were morphometrically quantified. Data obtained were statistically analyzed using the Variance method, and Tukey's Test(POBJETIVO: Avaliar o efeito do laser de baixa intensidade sobre a contração da pseudocápsula que ocorre ao redor de implantes de silicone. MÉTODOS: 60 ratos machos divididos em dois grupos receberam implante de silicone. Grupo I: implante no subcutâneo da região dorsal, sem tratamento após a cirurgia; Grupo II: animais receberam sete sessões de irradiação com laser de baixa intensidade após o implante. Trinta, 60 e 180 dias após a cirurgia, foi feita a tonometria dos implantes, Em seguida, os animais foram sacrificados, removendo-se o material de estudo que foi preparado para exame histológico, avaliando-se morfometricamente a espessura da pseudocápsula e a reação inflamatória. A análise estatistica pela técnica da Análise de Variância e Teste de Tukey (P<0.0 5. RESULTADOS: Pressões significativamente menores foram encontradas nos animais do grupo Grupo II. O estudo histológico não mostrou diferença significativa entre os grupos, destacando-se apenas maior quantidade de vasos intumescidos no Grupo II. A espessura da pseudocápsula foi menor no Grupo II. CONCLUS
SOLID BODY ABLATION UNDER EXPOSURE TO ULTRA SHORT LASER PULSES: STUDY BY MOLECULAR DYNAMICS METHODS
Directory of Open Access Journals (Sweden)
D. S. Ivanov
2014-09-01
Full Text Available The process of laser ablation under the influence of ultra short laser pulses on metals is investigated by methods of molecular dynamics. The validity and applicability of the hybrid atomistic-continuous model for the estimation of optimum modes of ultra short laser pulses processing are explored. Combination of atomistic model of laser-induced non-equilibrium process of a phase transition at the atomic level with continuous two-temperature model for describing the dynamics of photo-excitation of free media is proposed. Applicability of laser ablation model on the example of aluminum films and gold under exposure to pulses with different energy density and duration is shown. It is indicated that, depending on the ratio of the laser pulse duration and the characteristic time of electron-phonon material interaction, photothermal and photomechanical modes of destruction are implemented that determine the quality and performance of the laser processing. It is established that at the duration of laser pulse less than the time of electron-phonon interaction high-performance photomechanical type of destruction is implemented by internal stresses arising in the area of exposure. This is confirmed by a linear dependence of the ablation rate from the absorbed energy. At the duration of laser pulse greater than the time of electron-phonon interaction inefficient photothermal mode of destruction is implemented. The results may be useful for specialists engaged in the development of laser technologies
Signature of electron-phonon interaction in high temperature superconductors
Directory of Open Access Journals (Sweden)
Vinod Ashokan
2011-09-01
Full Text Available The theory of thermal conductivity of high temperature superconductors (HTS based on electron and phonon line width (life times formulation is developed with Quantum dynamical approach of Green's function. The frequency line width is observed as an extremely sensitive quantity in the transport phenomena of HTS as a collection of large number of scattering processes. The role of resonance scattering and electron-phonon interaction processes is found to be most prominent near critical temperature. The theory successfully explains the spectacular behaviour of high Tc superconductors in the vicinity of transition temperature. A successful agreement between theory and experiment has been obtained by analyzing the thermal conductivity data for the sample La1.8Sr0.2CuO4 in the temperature range 0 − 200K. The theory is equally and successfully applicable to all other high Tc superconductors.
Constitutive equation for polymer networks with phonon fluctuations.
Hansen, Rasmus; Skov, Anne Ladegaard; Hassager, Ole
2008-01-01
Recent research by Xing [Phys. Rev. Lett. 98, 075502 (2007)] has provided an expression for the Helmholtz free energy related to phonon fluctuations in polymer networks. We extend this result by constructing the corresponding nonlinear constitutive equation, usable for entirely general, volume conserving deformation fields. Constitutive equations for the sliplink model and the tube model are derived and the three models are examined by comparison with each other and with data from Xu and Mark [Rubber Chem. Technol. 63, 276 (1990)] and Wang and Mark [J. Polym. Sci., Part B: Polym. Phys. 30, 801 (1992)]. Elastic moduli are derived for the three models and compared with the moduli determined from the chemical stoichiometry. We conclude that the sliplink model and the phonon fluctuation model are relatively consistent with each other and with the data. The tube model seems consistent neither with the other models nor with the data.
Stochastic Approach to Phonon-Assisted Optical Absorption
Zacharias, Marios; Patrick, Christopher E.; Giustino, Feliciano
2015-10-01
We develop a first-principles theory of phonon-assisted optical absorption in semiconductors and insulators which incorporates the temperature dependence of the electronic structure. We show that the Hall-Bardeen-Blatt theory of indirect optical absorption and the Allen-Heine theory of temperature-dependent band structures can be derived from the present formalism by retaining only one-phonon processes. We demonstrate this method by calculating the optical absorption coefficient of silicon using an importance sampling Monte Carlo scheme, and we obtain temperature-dependent line shapes and band gaps in good agreement with experiment. The present approach opens the way to predictive calculations of the optical properties of solids at finite temperature.
Quantum Kinetic Theory and Applications Electrons, Photons, Phonons
Vasko, Fedir T
2006-01-01
This lecture-style monograph is addressed to several categories of readers. First, it will be useful for graduate students studying theory. Second, the topics covered should be interesting for postgraduate students of various specializations. Third, the researchers who want to understand the background of modern theoretical issues in more detail can find a number of useful results here. The phenomena covered involve kinetics of electron, phonon, and photon systems in solids. The dynamical properties and interactions of electrons, phonons, and photons are briefly described in Chapter 1. Further, in Chapters 2-8, the authors present the main theoretical methods: linear response theory, various kinetic equations for the quasiparticles under consideration, and diagram technique. The presentation of the key approaches is always accompanied by solutions of concrete problems to illustrate ways to apply the theory. The remaining chapters are devoted to various manifestations of quantum transport in solids. The choice...
Band structures in Sierpinski triangle fractal porous phononic crystals
Energy Technology Data Exchange (ETDEWEB)
Wang, Kai; Liu, Ying, E-mail: yliu5@bjtu.edu.cn; Liang, Tianshu
2016-10-01
In this paper, the band structures in Sierpinski triangle fractal porous phononic crystals (FPPCs) are studied with the aim to clarify the effect of fractal hierarchy on the band structures. Firstly, one kind of FPPCs based on Sierpinski triangle routine is proposed. Then the influence of the porosity on the elastic wave dispersion in Sierpinski triangle FPPCs is investigated. The sensitivity of the band structures to the fractal hierarchy is discussed in detail. The results show that the increase of the hierarchy increases the sensitivity of ABG (Absolute band gap) central frequency to the porosity. But further increase of the fractal hierarchy weakens this sensitivity. On the same hierarchy, wider ABGs could be opened in Sierpinski equilateral triangle FPPC; whilst, a lower ABG could be opened at lower porosity in Sierpinski right-angled isosceles FPPCs. These results will provide a meaningful guidance in tuning band structures in porous phononic crystals by fractal design.
Dynamics of vortices in neutral superfluids with noninteracting phonons
Fortin, Jean-Yves
2001-05-01
The transverse force on an isolated and moving vortex in a neutral superfluid at rest is evaluated at finite temperature in the case of noninteracting phonons. Using the Thouless, Ao, Niu (TAN) [Phys. Rev. Lett. 76, 3758 (1996)] general theory, we show that the transverse force is exactly equal to the superfluid Magnus force. We extend this theory in the case of a slowly moving vortex on a circular trajectory, and find an additional contribution coming from the centrifugal reaction. This term gives a negative vortex mass due to the phonons and diverges logarithmically at low frequency. The friction force is also evaluated for zero and finite frequencies, and compared with the scattering theory.
Exciton-Phonon Dynamics with Long-Range Interaction
Laskin, Nick
2011-01-01
Exciton-phonon dynamics on a 1D lattice with long-range exciton-exciton interaction have been introduced and elaborated. Long-range interaction leads to a nonlocal integral term in the motion equation of the exciton subsystem if we go from discrete to continuous space. In some particular cases for power-law interaction, the integral term can be expressed through a fractional order spatial derivative. A system of two coupled equations has been obtained, one is a fractional differential equation for the exciton subsystem, the other is a standard differential equation for the phonon subsystem. These two equations present a new fundamental framework to study nonlinear dynamics with long-range interaction. New approaches to model the impact of long-range interaction on nonlinear dynamics are: fractional generalization of Zakharov system, Hilbert-Zakharov system, Hilbert-Ginzburg-Landau equation and nonlinear Hilbert-Schrodinger equation. Nonlinear fractional Schrodinger equation and fractional Ginzburg-Landau equa...
Band gap tunability of magneto-elastic phononic crystal
Bou Matar, O.; Robillard, J. F.; Vasseur, J. O.; Hladky-Hennion, A.-C.; Deymier, P. A.; Pernod, P.; Preobrazhensky, V.
2012-03-01
The possibility of control and tuning of the band structures of phononic crystals offered by the introduction of an active magnetoelastic material and the application of an external magnetic field is studied. Two means to obtain large elastic properties variations in magnetoelastic material are considered: Giant magnetostriction and spin reorientation transition effects. A plane wave expansion method is used to calculate the band structures. The magnetoelastic coupling is taken into account through the consideration of an equivalent piezomagnetic material model with elastic, piezomagnetic, and magnetic permeability tensors varying as a function of the amplitude and orientation of the applied magnetic field. Results of contactless tunability of the absolute bandgap are presented for a two-dimensional phononic crystal constituted of Terfenol-D square rod embedded in an epoxy matrix.
Disclosing phonon squeezing by non-equilibrium optical experiments
Esposito, Martina; Zimmermann, Klaus; Giusti, Francesca; Randi, Francesco; Boschetto, Davide; Parmigiani, Fulvio; Floreanini, Roberto; Benatti, Fabio; Fausti, Daniele
2015-01-01
Fluctuations of the atomic positions are at the core of a large class of unusual material properties ranging from quantum para-electricity and charge density wave to, possibly, high temperature superconductivity. Their measurement in solids is subject of an intense scientific debate focused on the research of a methodology capable of establishing a direct link between the variance of the ionic displacements and experimentally measurable observables. Here we address this issue by means of non-equilibrium optical experiments performed in shot-noise limited regime. The variance of the time dependent atomic positions and momenta is directly mapped into the quantum fluctuations of the photon number of the scattered probing light. A fully quantum description of the non-linear interactions between photonic and phononic fields unveils evidences of squeezing of thermal phonons in $\\alpha-$quartz.
Lumped model for rotational modes in phononic crystals
Peng, Pai
2012-10-16
We present a lumped model for the rotational modes induced by the rotational motion of individual scatterers in two-dimensional phononic crystals comprised of square arrays of solid cylindrical scatterers in solid hosts. The model provides a physical interpretation of the origin of the rotational modes, reveals the important role played by the rotational motion in determining the band structure, and reproduces the dispersion relations in a certain range. The model increases the possibilities of manipulating wave propagation in phononic crystals. In particular, expressions derived from the model for eigenfrequencies at high symmetry points unambiguously predict the presence of a new type of Dirac-like cone at the Brillouin center, which is found to be the result of accidental degeneracy of the rotational and dipolar modes.
Coupling between the Magnetic Excitations and the Phonons in Praseodymium
DEFF Research Database (Denmark)
Jensen, J.
1976-01-01
The dispersion relation of the magnetic excitations of the hexagonal ions in DHCP Pr and the selection rules for the linear coupling to the phonons are determined by general symmetry considerations. The magnetic excitations propagating in the symmetry directions are considered in the cases...... of an external magnetic field applied along an a and a b direction. The magnetic excitations are approximated by pseudo-boson excitations of the spin sub-space, J=4, MJ=0 and +or-1, and the presence of the ions on the cubic sites is neglected. The selection rules deduced agree with experimental observations....... The experimental result for the strength of the exciton-phonon interaction is used in an estimate of the effects of an applied field on the elastic constants of Pr at zero temperature....
Plasmon-phonon coupling in graphene-hyperbolic bilayer heterostructures
Yin, Ge; Yuan, Jun; Jiang, Wei; Zhu, Jianfei; Ma, Yungui
2016-11-01
Polar dielectrics are important optical materials enabling the subwavelength manipulation of light in infrared due to their capability to excite phonon polaritons. In practice, it is highly desired to actively modify these hyperbolic phonon polaritons (HPPs) to optimize or tune the response of the device. In this work, we investigate the plasmonic material, a monolayer graphene, and study its hybrid structure with three kinds of hyperbolic thin films grown on SiO2 substrate. The inter-mode hybridization and their tunability have been thoroughly clarified from both the band dispersions and the mode patterns numerically calculated through a transfer matrix method. Our results show that these hybrid multilayer structures are of strong potentials for applications in plasmonic waveguides, modulators and detectors in infrared. Project supported by the National Natural Science Foundation of China (Grant No. 61271085) and the Natural Science Foundation of Zhejiang Province, China (Grant No. LR15F050001).
Extreme electron-phonon coupling in magnetic rubidium sesquioxide
de Groot, Robert; Attema, Jisk; Riyadi, S.; Blake, Greame; de Wijs, Gilles; Palstra, Thomas
2008-03-01
Rb2O3 is a black, opaque oxide. Early work suggests that the stability range of the sesquioxide phase in the rubidium-oxygen phase diagram is rather broad. Rb2O3 remains cubic down to the lowest temperature measured (5 K). The oxygens form dumbbells with interatomic distances in between those of peroxide and superoxide anions, and strong athermal motion persists down to low temperatures. [1] Electronic-structure calculations show that the dynamics at low temperature is caused by 6 phonon modes of zero frequency, which induce a very strong electron-phonon interaction. The softness of half of these modes is suppressed by the application of pressure. Calculated using the average oxygen positions, rubidium sesquioxide is a half-metallic ferromagnet. [2] [1] CR CHIM (11-13): 591-594 NOV 1999[2] JACS 127 (46): 16325-16328 NOV 23 2005
Nonlinear control of high-frequency phonons in spider silk
Schneider, Dirk; Gomopoulos, Nikolaos; Koh, Cheong Y.; Papadopoulos, Periklis; Kremer, Friedrich; Thomas, Edwin L.; Fytas, George
2016-10-01
Spider dragline silk possesses superior mechanical properties compared with synthetic polymers with similar chemical structure due to its hierarchical structure comprised of partially crystalline oriented nanofibrils. To date, silk’s dynamic mechanical properties have been largely unexplored. Here we report an indirect hypersonic phononic bandgap and an anomalous dispersion of the acoustic-like branch from inelastic (Brillouin) light scattering experiments under varying applied elastic strains. We show the mechanical nonlinearity of the silk structure generates a unique region of negative group velocity, that together with the global (mechanical) anisotropy provides novel symmetry conditions for gap formation. The phononic bandgap and dispersion show strong nonlinear strain-dependent behaviour. Exploiting material nonlinearity along with tailored structural anisotropy could be a new design paradigm to access new types of dynamic behaviour.
Phonons on the clean metal surfaces and in adsorption structures
Rusina, Galina G.; Chulkov, Evgenii V.
2013-06-01
The state-of-the-art studies of the vibrational dynamics of clean metal surfaces and metal surface structures formed upon the sub-monolayer adsorption of the atoms of various elements are considered. A brief historical survey of the milestones of investigations of surface phonons is presented. The results of studies of the atomic structure and vibration characteristics of surfaces with low and high Miller indices and adsorption structures are analyzed. It is demonstrated that vicinal surfaces of FCC metals tend to exhibit specific vibrational modes located on the step and polarized along the step. Irrespective of the type and position of adsorption or the substrate structure, the phonon spectra of sub-monolayer adsorption structures always tend to display two modes for combined translational displacements of adatoms and for coupled vibrations of substrate atoms and adatoms polarized in the direction normal to the surface. The bibliography includes 202 references.
Electron and phonon properties and gas storage in carbon honeycomb
Gao, Yan; Zhong, Chengyong; Zhang, Zhongwei; Xie, Yuee; Zhang, Shengbai
2016-01-01
A new kind of three-dimensional carbon allotropes, termed carbon honeycomb (CHC), has recently been synthesized [PRL 116, 055501 (2016)]. Based on the experimental results, a family of graphene networks are constructed, and their electronic and phonon properties are calculated by using first principles methods. All networks are porous metal with two types of electron transport channels along the honeycomb axis and they are isolated from each other: one type of channels is originated from the orbital interactions of the carbon zigzag chains and is topologically protected, while the other type of channels is from the straight lines of the carbon atoms that link the zigzag chains and is topologically trivial. The velocity of the electrons can reach ~106 m/s. Phonon transport in these allotropes is strongly anisotropic, and the thermal conductivities can be very low when compared with graphite by at least a factor of 15. Our calculations further indicate that these porous carbon networks possess high storage capa...
Thermodynamic potential of electrons and phonons system of disordered alloy
Repetskij, S P
2002-01-01
The cluster decomposition for the delayed two-time Green functions and the disordered crystal dynamic potential is obtained with an account of the electron-phonon and electron-electron interactions. The system electron states are described within the frames of the multizone strong coupling model. The calculations are based on the diagram technique for the Green temperature functions. The coherent potential approximation is chosen as the zero mononode approximation in this cluster decomposition method. It is shown that the processes of the contributions of the elementary excitations scattering on the clusters decrease with the cluster nodes number growth in the cluster in correspondence with certain small parameters. The analytical evaluations of the electron-phonon interaction impact on the electron energy spectrum of the ordering alloy are made in the monozone model. The possibility of applying the obtained results for describing the strong electron correlations impact on the electron structure and propertie...
Structural and phonon transmission study of Ge-Au-Ge eutectically bonded interfaces
Energy Technology Data Exchange (ETDEWEB)
Knowlton, W.B. [Univ. of California, Berkeley, CA (United States). Dept. of Materials Science and Mineral Engineering]|[Lawrence Berkeley Lab., CA (United States). Materials Sciences Div.
1995-07-01
This thesis presents a structural analysis and phonon transparency investigation of the Ge-Au-Ge eutectic bond interface. Interface development was intended to maximize the interfacial ballistic phonon transparency to enhance the detection of the dark matter candidate WIMPs. The process which was developed provides an interface which produces minimal stress, low amounts of impurities, and insures Ge lattice continuity through the interface. For initial Au thicknesses of greater than 1,000 {angstrom} Au per substrate side, eutectic epitaxial growth resulted in a Au dendritic structure with 95% cross sectional and 90% planar Au interfacial area coverages. In sections in which Ge bridged the interface, lattice continuity across the interface was apparent. Epitaxial solidification of the eutectic interface with initial Au thicknesses < 500 A per substrate side produced Au agglomerations thereby reducing the Au planar interfacial area coverage to as little as 30%. The mechanism for Au coalescence was attributed to lateral diffusion of Ge and Au in the liquid phase during solidification. Phonon transmission studies were performed on eutectic interfaces with initial Au thicknesses of 1,000 {angstrom}, 500 {angstrom}, and 300 {angstrom} per substrate side. Phonon imaging of eutectically bonded samples with initial Au thicknesses of 300 {angstrom}/side revealed reproducible interfacial percent phonon transmissions from 60% to 70%. Line scan phonon imaging verified the results. Phonon propagation TOF spectra distinctly showed the predominant phonon propagation mode was ballistic. This was substantiated by phonon focusing effects apparent in the phonon imaging data. The degree of interface transparency to phonons and resulting phonon propagation modes correlate with the structure of the interface following eutectic solidification. Structural studies of samples with initial Au thickness of 1,000 {angstrom}/side appear to correspond with the phonon transmission study.
McGinness, Lachlan P.; Savage, C. M.
2016-09-01
More than a decade ago, Edwin Taylor issued a "call to action" that presented the case for basing introductory university mechanics teaching around the principle of stationary action [E. F. Taylor, Am. J. Phys. 71, 423-425 (2003)]. We report on our response to that call in the form of an investigation of the teaching and learning of the stationary action formulation of physics in a first-year university course. Our action physics instruction proceeded from the many-paths approach to quantum physics to ray optics, classical mechanics, and relativity. Despite the challenges presented by action physics, students reported it to be accessible, interesting, motivational, and valuable.
Phonon amplification using evaporation and adsorption of helium
Energy Technology Data Exchange (ETDEWEB)
More, T.; Adams, J.S.; Bandler, S.R.; Broueer, S.M.; Lanou, R.E.; Maris, H.J.; Seidel, G.M. [Department of Physics, Brown University, Providence, Rhode Island 02912 (United States)
1996-07-01
We report the results of experiments designed to investigate the feasibility of amplifying a phonon signal using the evaporation of helium from a superfluid film and its subsequent readsorption onto a helium-free surface. We envision a multistage amplifier in which helium is evaporated from a wafer with a helium film only on one side and then adsorbed onto the film-free surface of a similar wafer. The phonons created by the adsorption reach the film on the opposite side of the wafer and potentially desorb more helium than was evaporated by the first wafer. The amplification would come from the high ratio of the binding energy of a helium atom to a film-free surface relative to the binding energy to the liquid. A number of experiments are reported that investigate the efficiencies of the individual steps of the process. The gain per stage is found to be about 3 for high-energy densities in which multiphonon processes are possible. At low-energy densities, the energy deposited into a film-free wafer is found to be less than the original input energy, with the ratio of output to input energy 0.2. Since in applications requiring amplification the phonon density produced by the adsorption of helium on a wafer will be low, the configuration we have studied{emdash}phonons produced in silicon coated with a saturated {sup 4}He film{emdash}will not result in amplification. However, other configurations might improve the efficiency enough to make an amplifier possible. {copyright} {ital 1996 The American Physical Society.}
Phonon spectrum, mechanical and thermophysical properties of thorium carbide
Energy Technology Data Exchange (ETDEWEB)
Pérez Daroca, D., E-mail: pdaroca@tandar.cnea.gov.ar [Gerencia de Investigación y Aplicaciones, Comisión Nacional de Energía Atómica (Argentina); Consejo Nacional de Investigaciones Cientı´ficas y Técnicas (Argentina); Jaroszewicz, S. [Gerencia de Investigación y Aplicaciones, Comisión Nacional de Energía Atómica (Argentina); Instituto de Tecnología Jorge A. Sabato, UNSAM-CNEA (Argentina); Llois, A.M. [Gerencia de Investigación y Aplicaciones, Comisión Nacional de Energía Atómica (Argentina); Consejo Nacional de Investigaciones Cientı´ficas y Técnicas (Argentina); Mosca, H.O. [Gerencia de Investigación y Aplicaciones, Comisión Nacional de Energía Atómica (Argentina); Instituto de Tecnología Jorge A. Sabato, UNSAM-CNEA (Argentina)
2013-06-15
In this work, we study, by means of density functional perturbation theory and the pseudopotential method, mechanical and thermophysical properties of thorium carbide. These properties are derived from the lattice dynamics in the quasi-harmonic approximation. The phonon spectrum of ThC presented in this article, to the best authors’ knowledge, have not been studied, neither experimentally, nor theoretically. We compare mechanical properties, volume thermal expansion and molar specific capacities with previous results and find a very good agreement.
Phonons in slow motion: dispersion relations in ultrathin Si membranes.
Cuffe, John; Chávez, Emigdio; Shchepetov, Andrey; Chapuis, Pierre-Olivier; El Boudouti, El Houssaine; Alzina, Francesc; Kehoe, Timothy; Gomis-Bresco, Jordi; Dudek, Damian; Pennec, Yan; Djafari-Rouhani, Bahram; Prunnila, Mika; Ahopelto, Jouni; Sotomayor Torres, Clivia M
2012-07-11
We report the changes in dispersion relations of hypersonic acoustic phonons in free-standing silicon membranes as thin as ∼8 nm. We observe a reduction of the phase and group velocities of the fundamental flexural mode by more than 1 order of magnitude compared to bulk values. The modification of the dispersion relation in nanostructures has important consequences for noise control in nano- and microelectromechanical systems (MEMS/NEMS) as well as opto-mechanical devices.
Phonon spectrum of single-walled boron nitride nanotubes
Institute of Scientific and Technical Information of China (English)
Xiao Yang; Yan Xiao-Hong; Cao Jue-Xian; Mao Yu-Liang; Xiang Jun
2004-01-01
Based on a force constant model, we investigated the phonon spectrum and then specific heat of single-walled boron nitride nanotubes. The results show that the frequencies of Raman and infrared active modes decrease with increasing diameter in the low frequency, which is consistent with the results calculated by density functional theory.The fitting formulae for diameter and chirality dependence of specific heat at 300K are given.
The phonon dispersion of wurtzite CdSe
Widulle, F.; Kramp, S.; Pyka, N. M.; Göbel, A.; Ruf, T.; Debernardi, A.; Lauck, R.; Cardona, M.
1999-03-01
We have measured the phonon dispersion of wurtzite CdSe along overlineΓA by inelastic neutron scattering at room temperature. The sample was grown with the very weakly neutron absorbing isotope 116Cd and natural selenium. These experiments extend the picture so far obtained from earlier measurements on 114CdS and deliver more information on the accuracy of theoretical models. The experimental data are compared with ab initio and shell model calculations.
Directory of Open Access Journals (Sweden)
Luisa eSartori
2015-05-01
Full Text Available Complementary colors are color pairs which, when combined in the right proportions, produce white or black. Complementary actions refer here to forms of social interaction wherein individuals adapt their joint actions according to a common aim. Notably, complementary actions are incongruent actions. But being incongruent is not sufficient to be complementary (i.e., to complete the action of another person. Successful complementary interactions are founded on the abilities: (i to simulate another person’s movements, (ii to predict another person’s future action/s, (iii to produce an appropriate incongruent response which differ, while interacting, with observed ones, and (iv to complete the social interaction by integrating the predicted effects of one’s own action with those of another person. This definition clearly alludes to the functional importance of complementary actions in the perception–action cycle and prompts us to scrutinize what is taking place behind the scenes. Preliminary data on this topic have been provided by recent cutting-edge studies utilizing different research methods. This mini-review aims to provide an up-to-date overview of the processes and the specific activations underlying complementary actions.
Nonsymmorphic Phononic Metamaterials: shaping waves over multiple length scales
Koh, Cheongyang; Thomas, Edwin
2012-02-01
The vector nature of the phonon makes rational design of phononic metamaterials challenging, despite potential in unique wave propagation behavior, such as negative refraction and hyper-lensing. While most designs to date focus on the ``meta-atom'' (building block) design, their ``spatial arrangement'' (non-locality) is equally instrumental in dispersion engineering. Here, we present a generalized design framework (DF) for PMM design, utilizing both ``global'' and ``local'' symmetry concepts. We demonstrate, utilizing specific properties of nonsymmorphic plane groups, PMMs possessing i) a low-frequency in-plane complete spectral gap (ICSG) of 102% (CSG of 88%), ii) a set of polychromatic ICSGs totaling over 100% in normalized gap size. Within the same DF, we further integrate broken symmetry states (BSS) (edge states, waveguides, etc) with designed polarization, (de)localization and group velocities. In particular, we demonstrate how these BSS may be utilized to elucidate signatures of complex polarization fields through phonon-structure interactions, leading to interesting applications in elastic-wave imaging, as well as information retrieval by probing polarization states of scattering bodies over multiple scales.
Anharmonic phonons and the isotope effect in superconductivity
Energy Technology Data Exchange (ETDEWEB)
Crespi, V.H.; Cohen, M.L. (Department of Physics, University of California at Berkeley, Berkeley, CA (USA) Materials Sciences Division, Lawrence Berkeley Laboratory, Berkeley, CA (USA)); Penn, D.R. (National Institute of Standards and Technology, Gaithersburg, MD (USA))
1991-06-01
Anharmonic interionic potentials are examined in an Einstein model to study the unusual isotope-effect exponents for the high-{ital T}{sub {ital c}} oxides. The mass dependences of the electron-phonon coupling constant {lambda} and the average phonon frequency {radical}{l angle}{omega}{sup 2}{r angle} are computed from weighted sums over the oscillator levels. The isotope-effect exponent is depressed below 1/2 by either a double-well potential or a potential with positive quadratic and quartic parts. Numerical solutions of Schroedinger's equation for double-well potentials produce {lambda}'s in the range 1.5--4 for a material with a vanishing isotope-effect parameter {alpha}. However, low phonon frequencies limit {ital T}{sub {ital c}} to roughly 15 K. A negative quartic perturbation to a harmonic well can increase {alpha} above 1/2. In the extreme-strong-coupling limit, {alpha} is 1/2, regardless of anharmonicity.
Phonon softening and dispersion in EuTiO3
Ellis, David S.; Uchiyama, Hiroshi; Tsutsui, Satoshi; Sugimoto, Kunihisa; Kato, Kenichi; Ishikawa, Daisuke; Baron, Alfred Q. R.
2012-12-01
We measured phonon dispersion in single-crystal EuTiO3 using inelastic x-ray scattering. A structural transition to an antiferrodistortive phase was found at a critical temperature T0=287±1 K using powder and single-crystal x-ray diffraction. Clear softening of the zone boundary R-point q=(0.50.50.5) acoustic phonon shows this to be a displacive transition. The mode energy plotted against reduced temperature could be seen to nearly overlap that of SrTiO3, suggesting a universal scaling relation. Phonon dispersion was measured along Γ-X (000)→(0.500). Mode eigenvectors were obtained from a shell model consistent with the q dependence of intensity and energy, which also showed that the dispersion is nominally the same as in SrTiO3 at room temperature, but corrected for mass. The lowest-energy optical mode, determined to be of Slater character, softens approximately linearly with temperature until the 70-100 K range where the softening stops, and at low temperature, the mode disperses linearly near the zone center.
Phonon- and phason-type spherical inclusions in icosahedral quasicrystals
Wang Jian Bo; Wang Ren Hui; Gastaldi, J
2003-01-01
Analytical expressions are derived as a first-order approximation for the elastic displacement fields, including both phonon- and phason-type components, induced by spherical inclusions in icosahedral quasicrystals (IQCs). The phonon-type component obtained is the same as that for a spherical inclusion in conventional elastically isotropic crystals, while the expression for the phason-type displacement, which decreases with increasing distance r to the sphere centre as r sup - sup 1 , is derived for the first time. Three concrete cases are discussed. The phonon part of the analytical expressions has been used to simulate the black-white double-lobe contrasts in the x-ray topograph (XRT) images of the strain field around the pores in the AlPdMn IQCs. The analytical expression for the phason-type displacement is used to simulate the XRT images of the strain field around spherical inclusions having isomorphic structures. The striking resemblance between experimental and simulated images suggests that such inclus...
Spin-phonon coupling in scandium doped gallium ferrite
Energy Technology Data Exchange (ETDEWEB)
Chakraborty, Keka R., E-mail: kekarc@barc.gov.in, E-mail: smyusuf@barc.gov.in; Mukadam, M. D.; Basu, S.; Yusuf, S. M., E-mail: kekarc@barc.gov.in, E-mail: smyusuf@barc.gov.in [Solid State Physics Division, Bhabha Atomic Research Centre, Mumbai 400085 (India); Paul, Barnita; Roy, Anushree [Department of Physics, Indian Institute of Technology, Kharagpur 721302 (India); Grover, Vinita; Tyagi, A. K. [Chemistry Division, Bhabha Atomic Research Centre, Mumbai 400085 (India)
2015-03-28
We embarked on a study of Scandium (Sc) doped (onto Ga site) gallium ferrite (GaFeO{sub 3}) and found remarkable magnetic properties. In both doped as well as parent compounds, there were three types of Fe{sup 3+} ions (depending on the symmetry) with the structure conforming to space group Pna2{sub 1} (Sp. Grp. No. 33) below room temperature down to 5 K. We also found that all Fe{sup 3+} ions occupy octahedral sites, and carry high spin moment. For the higher Sc substituted sample (Ga{sub 1−x}Sc{sub x}FeO{sub 3}: x = 0.3), a canted magnetic ordered state is found. Spin-phonon coupling below Néel temperature was observed in doped compounds. Our results indicated that Sc doping in octahedral site modifies spin-phonon interactions of the parent compound. The spin-phonon coupling strength was estimated for the first time in these Sc substituted compounds.
Stress Wave Isolation by Purely Mechanical Topological Phononic Crystals
Chaunsali, Rajesh; Li, Feng; Yang, Jinkyu
2016-08-01
We present an active, purely mechanical stress wave isolator that consists of short cylindrical particles arranged in a helical architecture. This phononic structure allows us to change inter-particle stiffness dynamically by controlling the contact angles of the cylinders. We use torsional travelling waves to control the contact angles, thereby imposing a desired spatio-temporal stiffness variation to the phononic crystal along the longitudinal direction. Such torsional excitation is a form of parametric pumping in the system, which results in the breakage of the time-reversal symmetry. We report that, in quasi-static sense, the system shows topologically non-trivial band-gaps. However, in a dynamic regime where the pumping effect is significant, these band-gaps become asymmetric with respect to the frequency and wavenumber domains in the dispersion relationship. By using numerical simulations, we show that such asymmetry has a direct correspondence to the topological invariant, i.e., Chern number, of the system. We propose that this asymmetry, accompanied by selective inter-band transition, can be utilized for directional isolation of the stress wave propagating along the phononic crystal.
Phonon impedance matching: minimizing interfacial thermal resistance of thin films
Polanco, Carlos; Zhang, Jingjie; Ghosh, Avik
2014-03-01
The challenge to minimize interfacial thermal resistance is to allow a broad band spectrum of phonons, with non-linear dispersion and well defined translational and rotational symmetries, to cross the interface. We explain how to minimize this resistance using a frequency dependent broadening matrix that generalizes the notion of acoustic impedance to the whole phonon spectrum including symmetries. We show how to ``match'' two given materials by joining them with a single atomic layer, with a multilayer material and with a graded superlattice. Atomic layer ``matching'' requires a layer with a mass close to the arithmetic mean (or spring constant close to the harmonic mean) to favor high frequency phonon transmission. For multilayer ``matching,'' we want a material with a broadening close to the geometric mean to maximize transmission peaks. For graded superlattices, a continuous sequence of geometric means translates to an exponentially varying broadening that generates a wide-band antireflection coating for both the coherent and incoherent limits. Our results are supported by ``first principles'' calculations of thermal conductance for GaAs / Gax Al1 - x As / AlAs thin films using the Non-Equilibrium Greens Function formalism coupled with Density Functional Perturbation Theory. NSF-CAREER (QMHP 1028883), NSF-IDR (CBET 1134311), XSEDE.
CO$_2$ Infrared Phonon Modes in Interstellar Ice Mixtures
Cooke, Ilsa R; Öberg, Karin I
2016-01-01
CO$_2$ ice is an important reservoir of carbon and oxygen in star and planet forming regions. Together with water and CO, CO$_2$ sets the physical and chemical characteristics of interstellar icy grain mantles, including desorption and diffusion energies for other ice constituents. A detailed understanding of CO$_2$ ice spectroscopy is a prerequisite to characterize CO$_2$ interactions with other volatiles both in interstellar ices and in laboratory experiments of interstellar ice analogs. We report laboratory spectra of the CO$_2$ longitudinal optical (LO) phonon mode in pure CO$_2$ ice and in CO$_2$ ice mixtures with H$_2$O, CO, O$_2$ components. We show that the LO phonon mode position is sensitive to the mixing ratio of various ice components of astronomical interest. In the era of JWST, this characteristic could be used to constrain interstellar ice compositions and morphologies. More immediately, LO phonon mode spectroscopy provides a sensitive probe of ice mixing in the laboratory and should thus enabl...
Squeezing properties of a trapped ion in the running-wave laser beyond the Lamb-Dicke limit
Institute of Scientific and Technical Information of China (English)
Pan Chang-Ning; Fang Mao-Fa; Zheng Xiao-Juan; Hu Yao-Hua
2007-01-01
Beyond the Lamb-Dicke limit, this paper investigates the squeezing properties of the trapped ion in the travelling-wave laser. It shows that the squeezing properties of the trapped ion in the travelling-wave laser are strongly affected by the sideband number k, the Lamb- Dicke parameterηand the initial average phonon number.
Yasuda, H.; Kubis, T.; Hosako, I.; Hirakawa, K.
2012-04-01
We theoretically investigated GaN-based resonant phonon terahertz-quantum cascade laser (QCL) structures for possible high-temperature operation by using the non-equilibrium Green's function method. It was found that the GaN-based THz-QCL structures do not necessarily have a gain sufficient for lasing, even though the thermal backfilling and the thermally activated phonon scattering are effectively suppressed. The main reason for this is the broadening of the subband levels caused by a very strong interaction between electrons and longitudinal optical (LO) phonons in GaN.
Gerecht, Eyal
NbN HEB mixers represent a promising approach for achieving receiver noise temperatures of a few times the quantum noise limit at frequencies above 1 THz. NbN HEB devices have been shown to have sufficient bandwidth for applications in astronomy, remote sensing, and plasma diagnostics in the FIR range. The NbN HEB is a phonon cooled bolometer in which the energy is transfered from the hot electrons to the substrate via inelastic collisions with phonons. The development of an NbN HEB mixer contained two steps: (1) implementing mixing in a comparatively large 'direct-coupled' prototype device which required LO power of a few milliwatts, and (2) optimization of the first step by the development of an 'antenna-coupled' (quasi-optically coupled) device with an LO power level of less than one μ W. The LO power was coupled to the antenna via an extended hemispherical lens (1.3 mm in diameter). The design, fabrication, and measurement stages were performed by a collaborative effort between a Russian team from the Department of Physics at Moscow State Pedagogical University in Moscow, the Submillimeter Technology Laboratory at UMass/Lowell and the Department of Electrical and Computer Engineering at UMass/Amherst. Mixing at 2.5 THz was demonstrated for the first time using the direct-coupled device achieving an intrinsic conversion loss of 23 dB. Sufficient level of LO power coupling at four different frequencies was demonstrated with the antenna-coupled device. The antenna/lens configuration has performed as well as expected insuring coupling to LO power of less than one μW. A 3 dB conversion gain was demonstrated with the antenna-coupled device using a laser LO at 1.56 THz with an IF frequency of 500 KHz. A second laser was utilized as the rf source. Noise temperature for the NbN HEB mixer receiver of 5800 K has been demonstrated over the 1.25-1.75 GHz IF band. The mixer temperature was 2500 K and the total conversion loss was 27 dB. Further optimization of the receiver
Spin-phonon coupling and ferroelectricity in magnetoelectric gallium ferrite
Mukherjee, Somdutta
2014-03-01
Gallium ferrite (GaFeO3 or GFO) is a low temperature ferrimagnet and room temperature piezoelectric wherein the magnetic transition temperature (TC) could be tailored to room temperature and above by tuning the stoichiometry and processing conditions. Such tunability of the magnetic transition temperature renders GFO a unique perspective in the research of multiferroics to potentially demonstrate room temperature magnetoelectric effect attractive for futuristic digital memory applications. Recent studies in several transition metal oxides highlight the importance of spin-phonon coupling in designing novel multiferroics by means of strain induced phase transition. In the present work, we have systematically studied the evolution of phonons in good quality samples of GFO across the TC using Raman spectroscopy. Using the phonon softening behavior and nearest neighbor spin-spin correlation function below TC we estimated spin-phonon coupling strength in the magnetically ordered state. In the process, we also show, for the first time, the presence of a spin glass phase in GFO where the spin-glass transition has a signature of abrupt change in spin-phonon coupling strength. Though GFO is piezoelectric and crystallizes in polar Pc21n symmetry, its ferroelectric nature remained controversial probably due to the large leakage current in the bulk material. To address this issue, we deposited epitaxial thin film on single crystalline yttria stabilized zirconia (YSZ) substrate using indium tin oxide (ITO) as a bottom conducting layer. We demonstrate clear evidence of room temperature ferroelectricity in the thin films from the 180o phase shift of the piezoresponse upon switching the electric field. Further, suppression of dielectric anomaly in presence of an external magnetic field clearly reveals a pronounced magneto-dielectric coupling across the magnetic transition temperature. In addition, using first principles calculations we elucidate that Fe ions are not only
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Coherent phonon decay and the boron isotope effect for MgB2.
Alarco, Jose A; Talbot, Peter C; Mackinnon, Ian D R
2014-12-14
Ab initio DFT calculations for the phonon dispersion (PD) and the phonon density of states (PDOS) of the two isotopic forms ((10)B and (11)B) of MgB2 demonstrate that use of a reduced symmetry super-lattice provides an improved approximation to the dynamical, phonon-distorted P6/mmm crystal structure. Construction of phonon frequency plots using calculated values for these isotopic forms gives linear trends with integer multiples of a base frequency that change in slope in a manner consistent with the isotope effect (IE). Spectral parameters inferred from this method are similar to that determined experimentally for the pure isotopic forms of MgB2. Comparison with AlB2 demonstrates that a coherent phonon decay down to acoustic modes is not possible for this metal. Coherent acoustic phonon decay may be an important contributor to superconductivity for MgB2.
Zhang, Yu; Yam, ChiYung; Chen, GuanHua
2015-04-28
A time-dependent inelastic electron transport theory for strong electron-phonon interaction is established via the equations of motion method combined with the small polaron transformation. In this work, the dissipation via electron-phonon coupling is taken into account in the strong coupling regime, which validates the small polaron transformation. The corresponding equations of motion are developed, which are used to study the quantum interference effect and phonon-induced decoherence dynamics in molecular junctions. Numerical studies show clearly quantum interference effect of the transport electrons through two quasi-degenerate states with different couplings to the leads. We also found that the quantum interference can be suppressed by the electron-phonon interaction where the phase coherence is destroyed by phonon scattering. This indicates the importance of electron-phonon interaction in systems with prominent quantum interference effect.
Energy Technology Data Exchange (ETDEWEB)
Zhang, Yu, E-mail: zhy@yangtze.hku.hk; Chen, GuanHua, E-mail: ghc@everest.hku.hk [Department of Chemistry, The University of Hong Kong, Pokfulam Road, Hong Kong (China); Yam, ChiYung [Department of Chemistry, The University of Hong Kong, Pokfulam Road, Hong Kong (China); Beijing Computational Science Research Center, Beijing 100084 (China)
2015-04-28
A time-dependent inelastic electron transport theory for strong electron-phonon interaction is established via the equations of motion method combined with the small polaron transformation. In this work, the dissipation via electron-phonon coupling is taken into account in the strong coupling regime, which validates the small polaron transformation. The corresponding equations of motion are developed, which are used to study the quantum interference effect and phonon-induced decoherence dynamics in molecular junctions. Numerical studies show clearly quantum interference effect of the transport electrons through two quasi-degenerate states with different couplings to the leads. We also found that the quantum interference can be suppressed by the electron-phonon interaction where the phase coherence is destroyed by phonon scattering. This indicates the importance of electron-phonon interaction in systems with prominent quantum interference effect.
Phonon blockade in a nanomechanical resonator resonantly coupled to a qubit
Xu, Xun-Wei; Liu, Yu-xi
2016-01-01
We study phonon statistics in a nanomechanical resonator (NAMR) which is resonantly coupled to a qubit. We find that there are two different mechanisms for phonon blockade in such a resonantly coupled NAMR-qubit system. One is due to the strong anharmonicity of the NAMR-qubit system with large coupling strength; the other one is due to the destructive interference between different paths for two-phonon excitation in the NAMR-qubit system with a moderate coupling strength. In order to enlarge the mean phonon number for strong phonon antibunching with a moderate NAMR-qubit coupling strength, we assume that two external driving fields are applied to the NAMR and qubit, respectively. In this case, we find that the phonon blockades under two mechanisms can appear at the same frequency regime by optimizing the strength ratio and phase difference of the two external driving fields.
Raman selection rule of surface optical phonon in ZnS nanobelts
Ho, Chih-Hsiang
2016-02-18
We report Raman scattering results of high-quality wurtzite ZnS nanobelts (NBs) grown by chemical vapor deposition. In Raman spectrum, the ensembles of ZnS NBs exhibit first order phonon modes at 274 cm-1 and 350 cm-1, corresponding to A1/E1 transverse optical and A1/E1 longitudinal optical phonons, in addition with strong surface optical (SO) phonon mode at 329 cm-1. The existence of SO band is confirmed by its shift with different surrounding dielectric media. Polarization dependent Raman spectrum was performed on a single ZnS NB and for the first time SO phonon band has been detected on a single nanobelt. Different selection rules of SO phonon modeshown from their corresponding E1/A1 phonon modeswere attributed to the anisotropic translational symmetry breaking on the NB surface.
A 1D Optomechanical crystal with a complete phononic band gap
Gomis-Bresco, J; Oudich, M; El-Jallal, S; Griol, A; Puerto, D; Chavez, E; Pennec, Y; Djafari-Rouhani, B; Alzina, F; Martínez, A; Torres, C M Sotomayor
2014-01-01
Recent years have witnessed the boom of cavity optomechanics, which exploits the confinement and coupling of optical waves and mechanical vibrations at the nanoscale. Amongst the different physical implementations,optomechanical (OM) crystals built on semiconductor slabs are particularly interesting since they enable the integration and manipulation of multiple OM elements in a single chip and provide GHz phonons suitable for coherent phonon manipulation. Different demonstrations of coupling of infrared photons and GHz phonons in cavities created by inserting defects on OM crystals have been performed. However, the considered structures do not show a complete phononic bandgap at the frequencies of interest, which in principle should allow longer dephasing time, since acoustic leakage is minimized. In this work we demonstrate the excitation of acoustic modes in a 1D OM crystal properly designed to display a full phononic bandgap for acoustic modes at about 4 GHz. The confined phonons have an OM coupling rangin...
New multi-phonon gamma vibrational bands in A～110 neutron-rich nuclei
Institute of Scientific and Technical Information of China (English)
HAMILTON; J; H; RAMAYYA; A; V; RASMUSSEN; J; O; HWANG; J; K; YEOH; E; Y
2011-01-01
The high spin states of neutron-rich 103Nb, 107Tc and 109Tc nuclei in A~110 region have been investigated by measuring prompt γ-γ-γ coincident measurements populated with the spontaneous fission of 252Cf with the Gammasphere detector array. In 103Nb, one-phonon K = 9/2 and two-phonon K = 13/2 γ-vibrational bands have been identified. In 107Tc and 109Tc, one-phonon K = 11/2 and two-phonon K = 15/2 γ-vibrational bands, in which the zero-phonon bands are based on K=7/2 excited states, have also been identified. The two-phonon bands are first observed in odd-Z nuclei. The characteristics for these band structures have been discussed.
Unified treatment of coupled optical and acoustic phonons in piezoelectric cubic materials
DEFF Research Database (Denmark)
Willatzen, Morten; Wang, Zhong Lin
2015-01-01
A unified treatment of coupled optical and acoustic phonons in piezoelectric cubic materials is presented whereby the lattice displacement vector and the internal ionic displacement vector are found simultaneously. It is shown that phonon couplings exist in pairs only; either between the electric...... potential and the lattice displacement coordinate perpendicular to the phonon wave vector or between the two other lattice displacement components. The former leads to coupled acousto-optical phonons by virtue of the piezoelectric effect. We then establish three new conjectures that entirely stem from...... piezoelectricity in a cubic structured material slab. First, it is shown that isolated optical phonon modes generally cannot exist in piezoelectric cubic slabs. Second, we prove that confined acousto-optical phonon modes only exist for a discrete set of in-plane wave numbers in piezoelectric cubic slabs. Third...
Phonon lifetime in SiSn and its suitability for hot-carrier solar cells
Energy Technology Data Exchange (ETDEWEB)
Levard, Hugo; Laribi, Sana; Guillemoles, Jean-François [Institute for Research and Development on Photovoltaic Energy (IRDEP), UMR 7174, EDF R and D/CNRS/Chimie ParisTech, 6 quai Watier, 78401 Chatou (France)
2014-06-02
We present a phononic and electronic study of SiSn in the zinc-blende phase. A detailed description of the longitudinal optical (LO) phonon decay in a three-phonon process is presented together with the corresponding lifetime. The necessity to go beyond the zone center phonon approximation in this case is highlighted as it reveals a steep dependence of the lifetime on the initial phonon wavenumber, which differs from usual semiconductors. The electronic band structure is calculated within the GW formalism and shows a small direct band gap. It is shown that the LO-phonon resulting from electron cooling has a lifetime four to eight orders of magnitude above all the known value in semiconductors for this process. We finally show the suitability of SiSn for hot-carrier solar cells, as it is endowed with ultra-slow cooling of hot carriers.
Short-pulse laser heating of metals: a new approach
Huettner, Bernd
1997-04-01
Recently, several groups have demonstrated that the spatial and temporal temperature distribution inside metals resulting from femtosecond laser pulses cannot be fully explained by the two-temperature model for the electrons and phonons. Since these short pulse lengths may be comparable to the electron temperature relaxation time, we introduce a heat flow which is nonlocal in time. By this way we are taking into account in first order a non-equilibrium distribution of the electrons. As a consequence, three additional terms appear in the differential equation for the electron temperature. Furthermore, we offer an explanation for the different response of metals to the laser radiation on the basis of the electron-phonon coupling constant and the average phonon frequencies squared, well-known quantities in McMillan's theory on superconductivity. Using a double temperature model with nonlocal heat flow and a laser pulse length of 1 ps, the calculated surface temperatures of the electron and phonon subsystems are presented for Cu, Nb, and Pb. This is compared with the results of a local heat flow approach and with the conventional theory as well. Additionally we present calculations of the electron surface temperature of a thin Au film. We find that our model is capable of describing the new measurements on Au films more consistently than the standard double temperature model.
Anharmonic effects in light scattering due to optical phonons in silicon
Balkanski, M.; Wallis, R. F.; Haro, E.
1983-08-01
Systematic measurements by light scattering of the linewidth and frequency shift of the q-->=0 optical phonon in silicon over the temperature range of 5-1400 K are presented. Both the linewidth and frequency shift exhibit a quadratic dependence on temperature at high temperatures. This indicates the necessity of including terms in the phonon proper self-energy corresponding to four-phonon anharmonic processes.
Ytterbium-driven strong enhancement of electron-phonon coupling in graphene
Hwang, Choongyu; Kim, Duck Young; Siegel, D. A.; Chan, Kevin T.; Noffsinger, J.; Fedorov, A. V.; Cohen, Marvin L.; Johansson, Börje; Neaton, J. B.; Lanzara, A.
2014-01-01
We present high-resolution angle-resolved photoemission spectroscopy study in conjunction with first principles calculations to investigate how the interaction of electrons with phonons in graphene is modified by the presence of Yb. We find that the transferred charges from Yb to the graphene layer hybridize with the graphene $\\pi$ bands, leading to a strong enhancement of the electron-phonon interaction. Specifically, the electron-phonon coupling constant is increased by as much as a factor ...
Jiang, Wanli; Feng, Duan; Xu, Dehui; Xiong, Bin; Wang, Yuelin
2016-10-01
In this paper, energy localization in line-defect resonator based on locally resonant phononic crystal (PnC) is experimentally studied. The defected resonator is realized by creating line defects on a two-dimension (2-D) silicon PnC. The silicon resonator was fabricated by micro machining process and tested by a combination of the fluid coupling method and Laser Doppler Vibrometer (LDV). Acoustic waves with frequency range from 7.19 MHz to 7.50 MHz are trapped in the cavity, and the corresponding resonant modes are observed in-situ. The measured quality (Q) factor of the resonator, which is 427 at its resonant frequency of 7.3 MHz, is smaller than the simulated ones (666 and 5135). The experimental results agree well with the simulation results that frequencies of the trapped acoustic waves of are mostly in the range of the phononic bandgaps. The locally resonant based PnC resonator in paper with 17 dB magnitude amplification, which is normalized with respect to the transmission of a freestanding silicon slab in the same frequency range, has great potential in energy harvesting or sound concentration.
Singh, Mahi R.; Brzozowski, Marek J.; Apter, Boris
2016-09-01
We investigate the light-matter interaction in a quantum emitter and metallic graphene flake (MGF) hybrid system deposited on a polar material. The coupling of surface plasmons in graphene and optical phonons in the polar material produces phonon-plasmon polaritons (PPPs). Similarly, couplings of photons with surface plasmons of graphene produce surface-plasmon polaritons (SPPs). Using the second quantized formulation for SPPs and PPPs interactions and density matrix method, we have calculated photoluminescence of the quantum emitters. It is found that when the exciton energy of the quantum emitter is in resonant with SPP and PPP energies, the photoluminescence in the quantum emitter are enhanced in the terahertz range. The enhancement is due to the transfer of SPP and PPP energies from the graphene flake to the quantum emitter. The energy transfer from graphene to the quantum emitter can be controlled by applying external pump lasers or stress and strain fields. These are interesting findings which can be used to fabricate switches and sensors.
Energy Technology Data Exchange (ETDEWEB)
Laguna, M.
1995-11-01
The electron machines`s development and improvement go through the discovery of new electron sources of high brightness. After reminding the interests in studying silicon cathodes with array of tips as electron sources, I describe, in the three steps model, the main phenomenological features related to photoemission and photoemission and photo-field-emission from a semi-conductor. the experimental set-ups used for the measurements reported in chapter four, five and six are described in chapter three. In chapter three. In chapter four several aspects of photo-field-emission in continuous and nanosecond regimes, studied on the Clermont-Ferrand`s test bench are tackled. We have measured quantum efficacies of 0.4 percent in the red (1.96 eV). Temporal responses in the nanoseconds range (10 ns) were observed with the Nd: YLF laser. With the laser impinging at an oblique angle we obtained ratios of photocurrent to dark current of the order of twenty. The issue of the high energy extracted photocurrent saturation is addressed and I give a preliminary explanation. In collaboration with the L.A.L. (Laboratoire de l`Accelerateur Lineaire) some tests with shortened pulsed laser beam (Nd: YAG laser 35 ps) were performed. Satisfactory response times have been obtained within the limitation of the scope (400 ps). (authors). 101 refs. 93 figs., 27 tabs., 3 photos., 1 append.
Raman probing of competitive laser heating and local recrystallization effect in ZnO nanocrystals.
Ye, J D; Parkinson, P; Ren, F F; Gu, S L; Tan, H H; Jagadish, C
2012-10-01
The competitive laser-induced local heating and recrystallization effects in ZnO nanocrystals embedded in a MgO/ZnO stack are reported via resonance Raman spectra. The dependence of the intensity, energy, and resonance effects of the longitudinal optical (LO) phonon on laser excitation condition are discussed in the context of Fröhlich interaction. Redistribution of defects, impurity-diffusion, and grain regrowth caused by thermal and photochemical effects lead to significant changes in coupling strength of electron-phonon interaction, and the resonance behaviors are strongly affected by the interplay of local heating, heat trapping, and local structural modification in such nanostructures.
Femtosecond laser crystallization of amorphous Ge
Salihoglu, Omer; Kürüm, Ulaş; Yaglioglu, H. Gul; Elmali, Ayhan; Aydinli, Atilla
2011-06-01
Ultrafast crystallization of amorphous germanium (a-Ge) in ambient has been studied. Plasma enhanced chemical vapor deposition grown a-Ge was irradiated with single femtosecond laser pulses of various durations with a range of fluences from below melting to above ablation threshold. Extensive use of Raman scattering has been employed to determine post solidification features aided by scanning electron microscopy and atomic force microscopy measurements. Linewidth of the Ge optic phonon at 300 cm-1 as a function of laser fluence provides a signature for the crystallization of a-Ge. Various crystallization regimes including nanostructures in the form of nanospheres have been identified.
Extended phonon collapse in the charge-density-wave compound NbSe{sub 2}
Energy Technology Data Exchange (ETDEWEB)
Weber, Frank [Karlsruhe Institute of Technology, Institute of Solid State Physics, Karlsruhe (Germany); Materials Science Division, Argonne National Laboratory, Argonne, Illinois (United States); Rosenkranz, Stephan; Castellan, John-Paul; Osborn, Raymond [Materials Science Division, Argonne National Laboratory, Argonne, Illinois (United States); Hott, Roland; Heid, Rolf; Bohnen, Klaus-Peter [Karlsruhe Institute of Technology, Institute of Solid State Physics, Karlsruhe (Germany); Egami, Takeshi [Department of Materials Science and Engineering, University of Tennessee, Knoxville, Tennessee (United States); Said, Ayman [Advanced Photon Source, Argonne National Laboratory, Illinois (United States); Reznik, Dmitry [Karlsruhe Institute of Technology, Institute of Solid State Physics, Karlsruhe (Germany); Department of Physics, University of Colorado at Boulder, Boulder, Colorado (United States)
2011-07-01
We investigated the phonon softening in the charge density wave compound NbSe{sub 2} using the high-resolution hard inelastic X-ray scattering beamline 30-ID-C at the Advanced Photon Source, Argonne National Laboratory. The acoustic {sigma}{sub 1} phonon branch was measured from the zone center {gamma} to the M point at temperatures between 250 K and 8 K across the CDW transition at T{sub CDW}=33 K. Density functional theory calculations for the lattice dynamical properties which predict an extended phonon breakdown are used to analyze the detailed nature of the softening phonon branch.
Non-markovian effects in semiconductor cavity QED: Role of phonon-mediated processes
DEFF Research Database (Denmark)
Nielsen, Per Kær; Nielsen, Torben Roland; Lodahl, Peter;
We show theoretically that the non-Markovian nature of the carrier-phonon interaction influences the dynamical properties of a semiconductor cavity QED system considerably, leading to asymmetries with respect to detuning in carrier lifetimes. This pronounced phonon effect originates from the pola......We show theoretically that the non-Markovian nature of the carrier-phonon interaction influences the dynamical properties of a semiconductor cavity QED system considerably, leading to asymmetries with respect to detuning in carrier lifetimes. This pronounced phonon effect originates from...
Acoustic phonons in the hexagonal perovskite CsNiCl3 around the Gamma-point
DEFF Research Database (Denmark)
Visser, D.; Monteith, A.R.; Rønnow, H.M.;
2000-01-01
The acoustic phonon dispersion curves of the hexagonal perovskite CsNiCl3 were measured at room temperature in the vicinity of the Gamma-point along the [0 0 1] and [1 1 0] directions. The derived velocity of sound values for the longitudinal and transverse acoustic phonons are compared with the ......The acoustic phonon dispersion curves of the hexagonal perovskite CsNiCl3 were measured at room temperature in the vicinity of the Gamma-point along the [0 0 1] and [1 1 0] directions. The derived velocity of sound values for the longitudinal and transverse acoustic phonons are compared...
Phonons in Solid Hydrogen and Deuterium Studied by Inelastic Coherent Neutron Scattering
DEFF Research Database (Denmark)
Nielsen, Mourits
1973-01-01
Phonon dispersion relations have been measured by coherent neutron scattering in solid para-hydrogen and ortho-deuterium. The phonon energies are found to be nearly equal in the two solids, the highest energy in each case lying close to 10 meV. The pressure and temperature dependence of the phonon...... energies have been measured in ortho-deuterium and the lattice change determined by neutron diffraction. When a pressure of 275 bar is applied, the phonon energies are increased by about 10%, and heating the crystal to near the melting point decreases them by about 7%. The densities of states, the specific...
Edge waves and resonances in two-dimensional phononic crystal plates
Hsu, Jin-Chen; Hsu, Chih-Hsun
2015-05-01
We present a numerical study on phononic band gaps and resonances occurring at the edge of a semi-infinite two-dimensional (2D) phononic crystal plate. The edge supports localized edge waves coupling to evanescent phononic plate modes that decay exponentially into the semi-infinite phononic crystal plate. The band-gap range and the number of edge-wave eigenmodes can be tailored by tuning the distance between the edge and the semi-infinite 2D phononic lattice. As a result, a phononic band gap for simultaneous edge waves and plate waves is created, and phononic cavities beside the edge can be built to support high-frequency edge resonances. We design an L3 edge cavity and analyze its resonance characteristics. Based on the band gap, high quality factor and strong confinement of resonant edge modes are achieved. The results enable enhanced control over acoustic energy flow in phononic crystal plates, which can be used in designing micro and nanoscale resonant devices and coupling of edge resonances to other types of phononic or photonic crystal cavities.
Theory of phonon properties in doped and undoped CuO nanoparticles
Bahoosh, S. G.; Apostolov, A. T.; Apostolova, I. N.; Wesselinowa, J. M.
2012-07-01
We have studied the phonon properties of CuO nanoparticles and have shown the importance of the anharmonic spin-phonon interaction. The Raman peaks of CuO nanoparticles shift to lower frequency and become broader as the particle size decreases in comparison with those of bulk CuO crystals owing to size effects. By doping with different ions, in dependence of their radius compared to the host ionic radius the phonon energies ω could be reduced or enhanced. The phonon damping is always enhanced through the ion doping effects.
Theory of phonon properties in doped and undoped CuO nanoparticles
Energy Technology Data Exchange (ETDEWEB)
Bahoosh, S.G. [Institute of Physics, Martin-Luther-University, D-06099 Halle (Germany); Apostolov, A.T. [University of Architecture, Civil Engineering and Geodesy Faculty of Hydrotechnics, Department of Physics, 1, Hristo Smirnenski Blvd., 1046 Sofia (Bulgaria); Apostolova, I.N. [University of Forestry, Faculty of Forest Industry, 10, Kl. Ohridsky Blvd., 1756 Sofia (Bulgaria); Wesselinowa, J.M., E-mail: julia@phys.uni-sofia.bg [University of Sofia, Department of Physics, 5 J. Bouchier Blvd., 1164 Sofia (Bulgaria)
2012-07-02
We have studied the phonon properties of CuO nanoparticles and have shown the importance of the anharmonic spin–phonon interaction. The Raman peaks of CuO nanoparticles shift to lower frequency and become broader as the particle size decreases in comparison with those of bulk CuO crystals owing to size effects. By doping with different ions, in dependence of their radius compared to the host ionic radius the phonon energies ω could be reduced or enhanced. The phonon damping is always enhanced through the ion doping effects. -- Highlights: ► The phonon properties of CuO nanoparticles are studied using a miscroscopic model. ► The phonon energy decreases whereas the damping increases with decreasing of particle size. ► It is shown the importance of the anharmonic spin–phonon interaction. ► By doping with RE-ions the phonon energy is reduced, whereas with TM-ions it is enhanced. ► The phonon damping is always enhanced through the ion doping effects.
PHONON-EXCITON MECHANISM IN YBa2Cu3O7-δ SYSTEM
Institute of Scientific and Technical Information of China (English)
Li Zhenji; Li Fengyue
2006-01-01
In this paper, based on the phonon-exciton mechanism, the superconductivity of yttrium barium copper oxide (YBCO) system is explained. The transition temperature (Tc) 's formula is derived by the extended BCS-Eliashberg theory, i.e. phonon-exciton mechanism and McMillan's energy gap function, and the Tc's expressions isreduced by using the Einstein spectrum. Last, the calculating method of element metal effective phonon spectrum is used to the high Tc cuprate YBCO system by using a crystal average atom approximation model. The theoretical analysis and calculational results show that the superconductivity of high Tc YBCO system maybe described by phonon-exciton model.
Superconductivity and electrical resistivity in alkali metal doped fullerides: Phonon mechanism
Indian Academy of Sciences (India)
Dinesh Varshney; A Dube; K K Choudhary; R K Singh
2005-04-01
We consider a two-peak model for the phonon density of states to investigate the nature of electron pairing mechanism for superconducting state in fullerides. We first study the intercage interactions between the adjacent C60 cages and expansion of lattice due to the intercalation of alkali atoms based on the spring model to estimate phonon frequencies from the dynamical matrix for the intermolecular alkali-C60 phonons. Electronic parameter as repulsive parameter and the attractive coupling strength are obtained within the random phase approximation. Transition temperature, c, is obtained in a situation when the free electrons in lowest molecular orbital are coupled with alkali-C60 phonons as 5 K, which is much lower as compared to reported c (≈ 20 K). The superconducting pairing is mainly driven by the high frequency intramolecular phonons and their effects enhance it to 22 K. To illustrate the usefulness of the above approach, the carbon isotope exponent and the pressure effect are also estimated. Temperature dependence of electrical resistivity is then analysed within the same model phonon spectrum. It is inferred from the two-peak model for phonon density of states that high frequency intramolecular phonon modes play a major role in pairing mechanism with possibly some contribution from alkali-C60 phonon to describe most of the superconducting and normal state properties of doped fullerides.
Band gaps and cavity modes in dual phononic and photonic strip waveguides
Directory of Open Access Journals (Sweden)
Y. Pennec
2011-12-01
Full Text Available We discuss theoretically the simultaneous existence of phoxonic, i.e., dual phononic and photonic, band gaps in a periodic silicon strip waveguide. The unit-cell of this one-dimensional waveguide contains a hole in the middle and two symmetric stubs on the sides. Indeed, stubs and holes are respectively favorable for creating a phononic and a photonic band gap. Appropriate geometrical parameters allow us to obtain a complete phononic gap together with a photonic gap of a given polarization and symmetry. The insertion of a cavity inside the perfect structure provides simultaneous confinement of acoustic and optical waves suitable to enhance the phonon-photon interaction.
Experimental evidence of zone-center optical phonon softening by accumulating holes in thin Ge
Energy Technology Data Exchange (ETDEWEB)
Kabuyanagi, Shoichi; Nishimura, Tomonori; Yajima, Takeaki; Toriumi, Akira [Department of Materials Engineering, The University of Tokyo, 7-3-1 Hongo, Tokyo 113-8656 (Japan)
2016-01-15
We discuss the impact of free carriers on the zone-center optical phonon frequency in germanium (Ge). By taking advantage of the Ge-on-insulator structure, we measured the Raman spectroscopy by applying back-gate bias. Phonon softening by accumulating holes in Ge film was clearly observed. This fact strongly suggests that the phonon softening in heavily-doped Ge is mainly attributed to the free carrier effect rather than the dopant atom counterpart. Furthermore, we propose that the free carrier effect on phonon softening is simply understandable from the viewpoint of covalent bonding modification by free carriers.
Surface optical phonon-assisted electron Raman scattering in a semiconductor quantum disc
Institute of Scientific and Technical Information of China (English)
刘翠红; 马本堃; 陈传誉
2002-01-01
We have carried out a theoretical calculation of the differential cross section for the electron Raman scatteringprocess associated with the surface optical phonon modes in a semiconductor quantum disc. Electron states are consid-ered to be confined within a quantum disc with infinite potential barriers. The optical phonon modes we have adoptedare the slab phonon modes by taking into consideration the Frohlich interaction between an electron and a phonon.The selection rules for the Raman process are given. Numerical results and a discussion are also presented for variousradii and thicknesses of the disc, and different incident radiation energies.
Nonlocal electron-phonon coupling in the pentacene crystal: Beyond the Γ-point approximation
Yi, Yuanping
2012-01-01
There is currently increasing interest in understanding the impact of the nonlocal (Peierls-type) electron-phonon mechanism on charge transport in organic molecular semiconductors. Most estimates of the non-local coupling constants reported in the literature are based on the Γ-point phonon modes. Here, the influence of phonon modes spanning the entire Brillouin zone (phonon dispersion) on the nonlocal electron-phonon couplings is investigated for the pentacene crystal. The phonon modes are obtained by using a supercell approach. The results underline that the overall nonlocal couplings are substantially underestimated by calculations taking sole account of the phonons at the Γ point of the unit cell. The variance of the transfer integrals based on Γ-point normal-mode calculations at room temperature is underestimated in some cases by 40% for herringbone-type dimers and by over 80% for cofacial dimers. Our calculations show that the overall coupling is somewhat larger for holes than for electrons. The results also suggest that the interactions of charge carriers (both electrons and holes) with acoustic and optical phonons are comparable. Therefore, an adequate description of the charge-transport properties in pentacene and similar systems requires that these two electron-phonon coupling mechanisms be treated on the same footing. © 2012 American Institute of Physics.
Korkusinski, M.; Studenikin, S. A.; Aers, G.; Granger, G.; Kam, A.; Sachrajda, A. S.
2017-02-01
Manipulating qubits via electrical pulses in a piezoelectric material such as GaAs can be expected to generate incidental acoustic phonons. In this Letter we determine theoretically and experimentally the consequences of these phonons for semiconductor spin qubits using Landau-Zener-Stückelberg interferometry. Theoretical calculations predict that phonons in the presence of the spin-orbit interaction produce both phonon-Rabi fringes and accelerated evolution at the singlet-triplet anticrossing. Observed features confirm the influence of these mechanisms. Additionally, evidence is found that the pulsed gates themselves act as phonon cavities increasing the influence of phonons under specific resonant conditions.
Kinetic approach for laser-induced heating of metals
Energy Technology Data Exchange (ETDEWEB)
Omar, Banaz; Rethfeld, Baerbel [Technical University of Kaiserslautern, Department of Physics, Erwin Schroedinger Str. 46, D-67663 Kaiserslautern (Germany)
2008-07-01
Non-equilibrium distribution functions of electron gas and phonon gas are calculated for metals irradiated with an ultrashort intense laser pulse. The excitation during femtosecond irradiation and the subsequent thermalization of the free electrons, as well as the dynamics of phonons can be described by a kinetic equation. The microscopic collision processes, such as absorption by inverse Bremsstrahlung, electron-electron, and electron-phonon interaction are considered with complete Boltzmann collision integrals. In contrast to aluminum, with a free-electron like conduction band considered in, the d-band in gold lies within the conduction band at about 2.5 eV below the Fermi surface of free electrons in s-band. Therefore, secondary electrons may be excited strongly, originating also from the d-band. We apply our kinetic approach to the case of gold by taking the electron density of states into account, and compare with the case of excitation of aluminum.
Identification of surface oxygen vacancy-related phonon-plasmon coupling in TiO2 single crystal
Guo, Jun-Hong; Li, Ting-Hui; Hu, Fang-Ren; Liu, Li-Zhe
2016-12-01
Oxygen vacancies (OVs) play a critical role in the physical properties and applications of titanium dioxide nanostructures, which are widely used in electrochemistry and photo catalysis nowadays. In this work, OVs were artificially introduced in the surface of a pure TiO2 single crystal by pulsed laser irradiation. Raman spectra showed that the intensity of Eg mode was enhanced. Theoretical calculations disclose that this was caused by the strong coupling effect between the phonon vibration and plasmon induced by the OVs-related surface deformation, and good agreement was achieved between the experiments and theory. Project supported by the National Natural Science Foundation of China (Grant Nos. 61574080, 11404162, 61505085, and 61264008) and the Natural Science Foundation of Jiangsu Province, China (Grant No. BK20130549).
Hong-Ou-Mandel interference of two phonons in trapped ions
Toyoda, Kenji; Hiji, Ryoto; Noguchi, Atsushi; Urabe, Shinji
2015-11-01
The quantum statistics of bosons and fermions manifest themselves in the manner in which two indistinguishable particles interfere quantum mechanically. When two photons, which are bosonic particles, enter a beam-splitter with one photon in each input port, they bunch together at either of the two output ports. The corresponding disappearance of the coincidence count is the Hong-Ou-Mandel effect. Here we show the phonon counterpart of this effect in a system of trapped-ion phonons, which are collective excitations derived by quantizing vibrational motions that obey Bose-Einstein statistics. We realize a beam-splitter transformation of the phonons by employing the mutual Coulomb repulsion between ions, and perform a two-phonon quantum interference experiment using that transformation. We observe an almost perfect disappearance of the phonon coincidence between two ion sites, confirming that phonons can be considered indistinguishable bosonic particles. The two-particle interference demonstrated here is purely a quantum effect, without a classical counterpart, hence it should be possible to demonstrate the existence of entanglement on this basis. We attempt to generate an entangled state of phonons at the centre of the Hong-Ou-Mandel dip in the coincidence temporal profile, under the assumption that the entangled phonon state is successfully generated if the fidelity of the analysis pulses is taken into account adequately. Two-phonon interference, as demonstrated here, proves the bosonic nature of phonons in a trapped-ion system. It opens the way to establishing phonon modes as carriers of quantum information in their own right, and could have implications for the quantum simulation of bosonic particles and analogue quantum computation via boson sampling.
Appavoo, Kannatassen; Wang, Bin; Brady, Nathaniel F; Seo, Minah; Nag, Joyeeta; Prasankumar, Rohit P; Hilton, David J; Pantelides, Sokrates T; Haglund, Richard F
2014-03-12
Ultrafast photoinduced phase transitions could revolutionize data-storage and telecommunications technologies by modulating signals in integrated nanocircuits at terahertz speeds. In quantum phase-changing materials (PCMs), microscopic charge, lattice, and orbital degrees of freedom interact cooperatively to modify macroscopic electrical and optical properties. Although these interactions are well documented for bulk single crystals and thin films, little is known about the ultrafast dynamics of nanostructured PCMs when interfaced to another class of materials as in this case to active plasmonic elements. Here, we demonstrate how a mesh of gold nanoparticles, acting as a plasmonic photocathode, induces an ultrafast phase transition in nanostructured vanadium dioxide (VO2) when illuminated by a spectrally resonant femtosecond laser pulse. Hot electrons created by optical excitation of the surface-plasmon resonance in the gold nanomesh are injected ballistically across the Au/VO2 interface to induce a subpicosecond phase transformation in VO2. Density functional calculations show that a critical density of injected electrons leads to a catastrophic collapse of the 6 THz phonon mode, which has been linked in different experiments to VO2 phase transition. The demonstration of subpicosecond phase transformations that are triggered by optically induced electron injection opens the possibility of designing hybrid nanostructures with unique nonequilibrium properties as a critical step for all-optical nanophotonic devices with optimizable switching thresholds.
Phonon Hall effect in four-terminal nano-junctions
Energy Technology Data Exchange (ETDEWEB)
Zhang Lifa; Wang Jiansheng; Li Baowen [Department of Physics and Centre for Computational Science and Engineering, National University of Singapore, 117546 Singapore (Singapore)], E-mail: phylibw@nus.edu.sg
2009-11-15
Using an exact nonequilibrium Green's function formulation, the phonon Hall effect (PHE) for paramagnetic dielectrics is studied in a nanoscale four-terminal device setting. The temperature difference in the transverse direction of the heat current is calculated for two-dimensional models with the magnetic field perpendicular to the plane. We find that there is a PHE in nanoscale paramagnetic dielectrics, the magnitude of which is comparable to millimeter scale experiments. If the dynamic matrix of the system satisfies mirror reflection symmetry, the PHE disappears. The Hall temperature difference changes sign if the magnetic field is sufficiently large or if the size increases.
Electron-phonon coupling in quasi free-standing graphene
DEFF Research Database (Denmark)
Christian Johannsen, Jens; Ulstrup, Søren; Bianchi, Marco;
2013-01-01
Quasi free-standing monolayer graphene can be produced by intercalating species like oxygen or hydrogen between epitaxial graphene and the substrate crystal. If the graphene is indeed decoupled from the substrate, one would expect the observation of a similar electronic dispersion and many......-body effects, irrespective of the substrate and the material used to achieve the decoupling. Here we investigate the electron-phonon coupling in two different types of quasi free-standing monolayer graphene: decoupled from SiC via hydrogen intercalation and decoupled from Ir via oxygen intercalation. Both...
Band structures in the nematic elastomers phononic crystals
Yang, Shuai; Liu, Ying; Liang, Tianshu
2017-02-01
As one kind of new intelligent materials, nematic elastomers (NEs) represent an exciting physical system that combines the local orientational symmetry breaking and the entropic rubber elasticity, producing a number of unique physical phenomena. In this paper, the potential application of NEs in the band tuning is explored. The band structures in two kinds of NE phononic crystals (PCs) are investigated. Through changing NE intrinsic parameters, the influence of the porosity, director rotation and relaxation on the band structures in NE PCs are analyzed. This work is a meaningful try for application of NEs in acoustic field and proposes a new intelligent strategy in band turning.
Validation of Phonon Physics in the CDMS Detector Monte Carlo
McCarthy, K A; Anderson, A J; Brandt, D; Brink, P L; Cabrera, B; Cherry, M; Silva, E Do Couto E; Cushman, P; Doughty, T; Figueroa-Feliciano, E; Kim, P; Mirabolfathi, N; Novak, L; Partridge, R; Pyle, M; Reisetter, A; Resch, R; Sadoulet, B; Serfass, B; Sundqvist, K M; Tomada, A
2011-01-01
The SuperCDMS collaboration is a dark matter search effort aimed at detecting the scattering of WIMP dark matter from nuclei in cryogenic germanium targets. The CDMS Detector Monte Carlo (CDMS-DMC) is a simulation tool aimed at achieving a deeper understanding of the performance of the SuperCDMS detectors and aiding the dark matter search analysis. We present results from validation of the phonon physics described in the CDMS-DMC and outline work towards utilizing it in future WIMP search analyses.
Phonon and magnon heat transport and drag effects
Heremans, Joseph P.
2014-03-01
Thermoelectric generators and coolers constitute today's solid-state energy converters. The two goals in thermoelectrics research are to enhance the thermopower while simultaneously maintaining a high electrical conductivity of the same material, and to minimize its lattice thermal conductivity without affecting its electronic properties. Up to now the lattice thermal conductivity has been minimized by using alloy scattering and, more recently, nanostructuring. In the first part of the talk, a new approach to minimize the lattice thermal conductivity is described that affects phonon scattering much more than electron scattering. This can be done by selecting potential thermoelectric materials that have a very high anharmonicity, because this property governs phonon-phonon interaction probability. Several possible types of chemical bonds will be described that exhibit such high anharmonicity, and particular emphasis will be put on solids with highly-polarizable lone-pair electrons, such as the rock salt I-V-VI2 compounds (e.g. NaSbSe2). The second part of the talk will give an introduction to a completely new class of solid-state thermal energy converters based on spin transport. One configuration for such energy converters is based on the recently discovered spin-Seebeck effect (SSE). This quantity is expressed in the same units as the conventional thermopower, and we have recently shown that it can be of the same order of magnitude. The main advantage of SSE converters is that the problem of optimization is now distributed over two different materials, a ferromagnet in which a flux of magnetization is generated by a thermal gradient, and a normal metal where the flux of magnetization is converted into electrical power. The talk will focus on the basic physics behind the spin-Seebeck effect. Recent developments will then be described based on phonon-drag of spin polarized electrons. This mechanism has made it possible to reach magnitudes of SSE that are comparable
Optical phonon modes in rhombohedral boron monosulfide under high pressure
Energy Technology Data Exchange (ETDEWEB)
Cherednichenko, Kirill A. [Synchrotron SOLEIL, 91192 Gif-sur-Yvette (France); IMPMC, UPMC Sorbonne Universités, CNRS UMR 7590, 75005 Paris (France); LSPM–CNRS, Université Paris Nord, 93430 Villetaneuse (France); Sokolov, Petr S.; Solozhenko, Vladimir L., E-mail: vladimir.solozhenko@univ-paris13.fr [LSPM–CNRS, Université Paris Nord, 93430 Villetaneuse (France); Kalinko, Aleksandr [Synchrotron SOLEIL, 91192 Gif-sur-Yvette (France); Institute of Solid State Physics, University of Latvia, LV-1063 Riga (Latvia); Le Godec, Yann; Polian, Alain [IMPMC, UPMC Sorbonne Universités, CNRS UMR 7590, 75005 Paris (France); Itié, Jean-Paul [Synchrotron SOLEIL, 91192 Gif-sur-Yvette (France)
2015-05-14
Raman spectra of rhombohedral boron monosulfide (r-BS) were measured under pressures up to 34 GPa at room temperature. No pressure-induced structural phase transition was observed, while strong pressure shift of Raman bands towards higher wavenumbers has been revealed. IR spectroscopy as a complementary technique has been used in order to completely describe the phonon modes of r-BS. All experimentally observed bands have been compared with theoretically calculated ones and modes assignment has been performed. r-BS enriched by {sup 10}B isotope was synthesized, and the effect of boron isotopic substitution on Raman spectra was observed and analyzed.
Spectroscopy of phonons and spin torques in magnetic point contacts.
Yanson, I K; Naidyuk, Yu G; Bashlakov, D L; Fisun, V V; Balkashin, O P; Korenivski, V; Konovalenko, A; Shekhter, R I
2005-10-28
Phonon spectroscopy is used to investigate the mechanism of current-induced spin torques in nonmagnetic/ferromagnetic (N/F) point contacts. Magnetization excitations observed in the magneto-conductance of the point contacts are pronounced for diffusive and thermal contacts, where the electrons experience significant scattering in the contact region. We find no magnetic excitations in highly ballistic contacts. Our results show that impurity scattering at the N/F interface is the origin of the new single-interface spin torque effect.
Phonon assisted thermophoretic motion of gold nanoparticles inside carbon nanotubes
Schoen, Philipp A. E.; Walther, Jens H.; Poulikakos, Dimos; Koumoutsakos, Petros
2007-06-01
The authors investigate the thermally driven mass transport of gold nanoparticles confined inside carbon nanotubes using molecular dynamics simulations. The observed thermophoretic motion of the gold nanoparticles correlates with the phonon dispersion exhibited by a standard carbon nanotube and, in particular, with the breathing mode of the tube. Additionally, the results show an increased static friction for gold nanoparticles confines inside a zig-zag carbon nanotube when increasing the size (length) of the nanoparticles. However, an unexpected, opposite trend is observed for the same nanoparticles inside armchair tubes.